publicationDate,title,abstract,id 2008-04-26,Origin of resistivity minima at low temperature in ferromagnetic metallic manganites,"The resistivity and magnetoresistance measurements were carried out on thin film of La0.7Ca0.3MnO3 to investigate the possible origin of low temperature resistivity minimum observed in these samples. We observed large hysteresis in the magnetoresistance at low temperature; 5K and the sample current I has large effect on resistivity minima temperature. The observation of hysteresis at low temperatures suggests the presence of inhomogeneity at low temperatures. These in-homogeneities consist of regions of different resistive phases. It appears that the high resistive phase prevents the tunneling of charge carriers between two low resistive regions and thus giving rise to the resistivity minimum in these samples.",0804.4247v1 2015-08-05,The universal influence of contact resistance on the efficiency of a thermoelectric generator,"The influence of electrical and thermal contact resistance on the efficiency of a segmented thermoelectric generator is investigated. We consider 12 different segmented $p$-legs and 12 different segmented $n$-legs, using 8 different $p$-type and 8 different $n$-type thermoelectric materials. For all systems a universal influence of both the electrical and thermal contact resistance is observed on the leg's efficiency, when the systems are analyzed in terms of the contribution of the contact resistance to the total resistance of the leg. The results are compared with the analytical model of Min and Rowe (1992). In order for the efficiency not to decrease more than 20%, the contact electrical resistance should be less than 30% of the total leg resistance for zero thermal contact resistance, while the thermal contact resistance should be less than 20% for zero electrical contact resistance. The universal behavior also allowed the maximum tolerable contact resistance for a segmented system to be found, i.e. the resistance at which a leg of only the high temperature thermoelectric material has the same efficiency as the segmented leg with a contact resistance at the interface. If e.g. segmentation increases the efficiency by 30% then an electrical contact resistance of 30% or a thermal contact resistance of 20% can be tolerated.",1508.01153v1 2018-02-10,Electroforming Free Controlled Bipolar Resistive Switching in Al/CoFe2O4/FTO device with Self-Compliance Effect,"Controlled bipolar resistive switching (BRS) has been observed in nanostructured CoFe2O4 films using Al(aluminum)/CoFe2O4/FTO(fluorine-doped tin oxide) device. The fabricated device shows electroforming-free uniform BRS with two clearly distinguished and stable resistance states without any application of compliance current (CC), with a resistance ratio of high resistance state (HRS) and low resistance state (LRS) > 102. Small switching voltage (< 1 volt) and lower current in both the resistance states confirms the fabrication of low power consumption device. In the LRS, the conduction mechanism was found to be of Ohmic in nature, while the high-resistance state (HRS/OFF state) was governed by space charge-limited conduction mechanism, which indicates the presence of an interfacial layer with imperfect microstructure near the top Al/CFO interface. The device shows nonvolatile behavior with good endurance properties, acceptable resistance ratio, uniform resistive switching due to stable, less random filament formation/rupture and a control over the resistive switching properties by choosing different stop voltages, which makes the device suitable for its application in future nonvolatile resistive random access memory (ReRAM).",1802.03643v1 2021-08-20,Understanding grain boundary electrical resistivity in Cu: the effect of boundary structure,"Grain boundaries (GBs) in metals usually increase electrical resistivity due to their distinct atomic arrangement compared to the grain interior. While the GB structure has a crucial influence on the electrical properties, its relationship with resistivity is poorly understood. Here, we perform a systematic study on the resistivity and structure relationship in Cu tilt GBs, employing high resolution in-situ electrical measurements coupled with atomic structure analysis of the GBs. Excess volume and energies of selected GBs are calculated using molecular dynamics simulations. We find a consistent relation between the coincidence site lattice (CSL) type of the GB and its resistivity. The most resistive GBs are high range of low-angle GBs (misorientation 14 to 18 degrees) with twice the resistivity of high angle tilt GBs, due to the high dislocation density and corresponding strain fields. Regarding the atomistic structure, GB resistivity approximately correlates with the GB excess volume. Moreover, we show that GB curvature increases resistivity by about 80%, while phase variations and defects within the same CSL type do not considerably change it.",2108.09148v1 2003-12-07,Temperature-dependent contact resistances in high-quality polymer field-effect transistors,"Contact resistances between organic semiconductors and metals can dominate the transport properties of electronic devices incorporating such materials. We report measurements of the parasitic contact resistance and the true channel resistance in bottom contact poly(3-hexylthiophene) (P3HT) field-effect transistors with channel lengths from 400 nm up to 40 $\mu$m, from room temperature down to 77 K. For fixed gate voltage, the ratio of contact to channel resistance decreases with decreasing temperature. We compare this result with a recent model for metal-organic semiconductor contacts. Mobilities corrected for this contact resistance can approach 1 cm$^{2}$/Vs at room temperature and high gate voltages.",0312183v1 2024-02-26,A novel method for determining the resistivity of compressed superconducting materials,"The resistivity of a superconductor in its normal state plays a critical role in determining its superconducting ground state. However, measuring the resistivity of a material under high pressure has long presented a significant technical challenge due to pressure-induced changes in the crystallographic directions, especially for samples with anisotropic layered structures like high-Tc superconductors and other intriguing quantum materials. Here, we are the first to propose a novel and effective method for determining high-pressure resistivity, which relies on the ambient-pressure resistivity, initial sample sizes, lattice parameters, high-pressure resistance, and lattice parameters measured from the same sample. Its validity has been confirmed through our investigations of pressurized copper-oxide superconductors, which demonstrates that this method provides new possibilities for researchers conducting high-pressure studies related to resistivity of these materials.",2402.16257v1 2021-09-14,Internal reverse-biased p-n junctions: a possible origin of the high resistance in phase change superlattice,"Phase change superlattice is one of the emerging material technologies for ultralow-power phase change memories. However, the resistance switching mechanism of phase change superlattice is still hotly debated. Early electrical measurements and recent materials characterizations have suggested that the Kooi phase is very likely to be the as-fabricated low-resistance state. Due to the difficulty in in-situ characterization at atomic resolution, the structure of the electrically switched superlattice in its high-resistance state is still unknown and mainly investigated by theoretical modellings. So far, there has been no simple model that can unify experimental results obtained from device-level electrical measurements and atomic-level materials characterizations. In this work, we carry out atomistic transport modellings of the phase change superlattice device and propose a simple mechanism accounting for its high resistance. The modeled high-resistance state is based on the interfacial phase changed superlattice that has previously been mistaken for the low-resistance state. This work advances the understanding of phase change superlattice for emerging memory applications.",2109.06376v1 2018-04-23,Magnetic field-induced resistivity upturn and exceptional magneto-resistance in Weyl semimetal TaSb2,"We study magneto-transport properties in single crystals of TaSb_2, which is a recently discovered topological semimetal. In the presence of magnetic field, the electrical resistivity shows onset of insulating behaviour followed by plateau at low temperature. Such resistivity plateau is generally assigned to topological surface states. TaSb2 exhibits extremely high magneto-resistance with non-saturating field dependence. We find that aspects of extremely large magneto resistance and resistivity plateau are well accounted by classical Kohler scaling. Unambiguous evidence for anomalous Chiral transport is provided with observation of negative longitudinal magneto-resistance. Shubnikov-de Haas oscillations reveal two dominating frequencies, 201 T and 455 T. These aspects categorize TaSb2 as a Type-II Weyl semimetal. At low temperature, the field dependence of Hall resistivity shows non-linear behaviour that indicates the presence of two types of charge carriers in consonance with reported electronic band structure. Analysis of Hall resistivity imply very high electron mobilities.",1804.08434v1 2023-07-12,Machine learning accelerated discovery of corrosion-resistant high-entropy alloys,"Corrosion has a wide impact on society, causing catastrophic damage to structurally engineered components. An emerging class of corrosion-resistant materials are high-entropy alloys. However, high-entropy alloys live in high-dimensional composition and configuration space, making materials designs via experimental trial-and-error or brute-force ab initio calculations almost impossible. Here we develop a physics-informed machine-learning framework to identify corrosion-resistant high-entropy alloys. Three metrics are used to evaluate the corrosion resistance, including single-phase formability, surface energy and Pilling-Bedworth ratios. We used random forest models to predict the single-phase formability, trained on an experimental dataset. Machine learning inter-atomic potentials were employed to calculate surface energies and Pilling-Bedworth ratios, which are trained on first-principles data fast sampled using embedded atom models. A combination of random forest models and high-fidelity machine learning potentials represents the first of its kind to relate chemical compositions to corrosion resistance of high-entropy alloys, paving the way for automatic design of materials with superior corrosion protection. This framework was demonstrated on AlCrFeCoNi high-entropy alloys and we identified composition regions with high corrosion resistance. Machine learning predicted lattice constants and surface energies are consistent with values by first-principles calculations. The predicted single-phase formability and corrosion-resistant compositions of AlCrFeCoNi agree well with experiments. This framework is general in its application and applicable to other materials, enabling high-throughput screening of material candidates and potentially reducing the turnaround time for integrated computational materials engineering.",2307.06384v3 2014-08-26,Enhancement in Quality Factor of SRF Niobium Cavities by Material Diffusion,"An increase in the quality factor of superconducting radiofrequency cavities is achieved by minimizing the surface resistance during processing steps. The surface resistance is the sum of temperature independent residual resistance and temperature/material dependent Bardeen-Cooper-Schrieffer (BCS) resistance. High temperature heat treatment usually reduces the impurities concentration from the bulk niobium, lowering the residual resistance. The BCS part can be reduced by selectively doping non-magnetic impurities. The increase in quality factor, termed as Q-rise, was observed in cavities when titanium or nitrogen thermally diffused in the inner cavity surface.",1408.6245v1 2015-12-15,A Graphene-Carbon Nanotube Hybrid Material for Photovoltaic Applications,"Large area graphene sheets grown by chemical vapor deposition can potentially be employed as a transparent electrode in photovoltaics if their sheet resistance can be significantly lowered, without any loss in transparency. Here, we report the fabrication of a graphene-conducting-carbon-nanotube (CCNT) hybrid material with a sheet resistance considerably lower than neat graphene, and with the requisite small reduction in transparency. Graphene is deposited on top of a a self-assembled CCNT monolayer which creates parallel conducting paths on the graphene surface. The hybrid thereby circumvents electron scattering due to defects in the graphene sheet, and reduces the sheet resistance by a factor of two. The resistance can be further reduced by chemically doping the hybrid. Moreover, the chemically doped hybrid is more stable than a standalone chemically doped graphene sheet, as the CCNT network enhances the dopant binding. In order to understand the results, we develop a 2D resistance network model in which we couple the CCNT layer to the graphene sheet and demonstrate the model accounts quantitatively for the resistance decrease. Our results show that a graphene-CCNT hybrid system has high potential for use as a transparent electrode with high transparency and low sheet resistance.",1512.04617v1 2022-06-11,Modeling of High and Low Resistant States in Single Defect Atomristors,"Resistance-change random access memory (RRAM) devices are nanoscale metal-insulator-metal structures that can store information in their resistance states, namely the high resistance (HRS) and low resistance (LRS) states. They are a potential candidate for a universal memory as these non-volatile memory elements can offer fast-switching, long retention and switching cycles, and additionally, are also suitable for direct applications in neuromorphic computing. In this study, we first present a model to analyze different resistance states of RRAM devices or so-called ""atomristors"" that utilize novel 2D materials as the switching materials instead of insulators. The developed model is then used to study the electrical characteristics of a single defect monolayer MoS$_{2}$ memristor. The change in the device resistance between the HRS and LRS is associated to the change in the tunneling probability when the vacancy defects in the 2D material are substituted by the metal atoms from the electrodes. The distortion due to defects and substituted metal atom is captured in the 1D potential energy profile by averaging the effect along the transverse direction. This simplification enables us to model single defect memristors with a less extensive quantum transport model while taking into account the presence of defects.",2206.05504v1 2011-06-06,Efficient resistive memory effect on SrTiO3 by ionic-bombardment,"SrTiO3 is known to exhibit resistive memory effect either with cation-doping or with high-temperature thermal reduction. Here, we add another scheme, ionic-bombardment, to the list of tools to create resistive memory effect on SrTiO3 (STO). In an Ar-bombarded STO crystal, two orders of resistance difference was observed between the high and low resistive states, which is an order of magnitude larger than those achieved by the conventional thermal reduction process. One of the advantages of this new scheme is that it can be easily combined with lithographic processes to create spatially-selective memory effect.",1106.1203v1 2006-02-21,Evidance for an Oxygen Diffusion Model for the Electric Pulse Induced Resistance Change Effect in Oxides,"Electric pulse induced resistance (EPIR) switching hysteresis loops for Pr0.7Ca0.7MnO3 (PCMO) perovskite oxide films were found to exhibit an additional sharp ""shuttle peak"" around the negative pulse maximum for films deposited in an oxygen deficient ambient. The device resistance hysteresis loop consists of stable high resistance and low resistance states, and transition regions between them. The resistance relaxation of the ""shuttle peak"" and its temperature behavior as well as the resistance relaxation in the transition regions were studied, and indicate that the resistance switching relates to oxygen diffusion with activation energy about 0.4eV. An oxygen diffusion model with the oxygen ions (vacancies) as the active agent is proposed for the non-volatile resistance switching effect in PCMO.",0602507v2 2014-06-16,Degenerate Resistive Switching and Ultrahigh Density Storage in Resistive Memory,"We show that, in tantalum oxide resistive memories, activation power provides a multi-level variable for information storage that can be set and read separately from the resistance. These two state variables (resistance and activation power) can be precisely controlled in two steps: (1) the possible activation power states are selected by partially reducing resistance, then (2) a subsequent partial increase in resistance specifies the resistance state and the final activation power state. We show that these states can be precisely written and read electrically, making this approach potentially amenable for ultra-high density memories. We provide a theoretical explanation for information storage and retrieval from activation power and experimentally demonstrate information storage in a third dimension related to the change in activation power with resistance.",1406.4033v1 2020-06-10,Positive versus negative resistance response to hydrogenation in palladium and its alloys,"Resistive solid state sensors are widely used in multiple applications, including molecular and gas detection. Absorption or intercalation of the target species varies the lattice parameters and an effective thickness of thin films, which is usually neglected in analyzing their transport properties in general and the sensor response in particular. Here, we explore the case of palladium-based thin films absorbing hydrogen and demonstrate that expansion of thickness is an important mechanism determining the magnitude and the very polarity of the resistance response to hydrogenation in high resistivity films. The model of the resistance response that takes into account modifications of thickness was tested and confirmed in three Pd-based systems with variable resistivity: thin Pd films above and below the percolation threshold, thick Pd-SiO2 granular composite films with different content of silica, and Pd-rich CoPd alloys where resistivity depends on Co concentration. Superposition of the bulk resistivity increase due to hydride formation and decrease of film resistance due to thickness expansion provides a consistent explanation of the hydrogenation response in both continuous and discontinuous films with different structures and compositions.",2006.05801v1 2021-06-04,Noncured Graphene Thermal Interface Materials: Minimizing the Thermal Contact Resistance,"We report on experimental investigation of thermal contact resistance of the noncuring graphene thermal interface materials with the surfaces characterized by different degree of roughness. It is found that the thermal contact resistance depends on the graphene loading non-monotonically, achieving its minimum at the loading fraction of ~15 wt.%. Increasing the surface roughness by ~1 micrometer results in approximately the factor of x2 increase in the thermal contact resistance for this graphene loading. The obtained dependences of the thermal conductivity, thermal contact resistance, and the total thermal resistance of the thermal interface material layer on the graphene loading and surface roughness indicate the need for optimization of the loading fraction for specific materials and roughness of the connecting surfaces. Our results are important for developing graphene technologies for thermal management of high-power-density electronics.",2106.02180v1 2002-10-24,Violation of Ioffe-Regel condition but saturation of resistivity of the high Tc cuprates,"We demonstrate that the resistivity data of a number of high Tc cuprates, in particular La(2-x)SrxCuO4, are consistent with resistivity saturation, although the Ioffe-Regel condition is strongly violated. By using the f-sum rule together with calculations of the kinetic energy in the t-J model, we show that the saturation resistivity is unusually large. This is related to the strong reduction of the kinetic energy due to strong correlation effects. The fulfilment of the Ioffe-Regel condition for conventional transition metal compounds is found to be somewhat accidental.",0210543v1 2023-04-26,Theoretical Puncture Mechanics of Soft Compressible Solids,"Accurate prediction of the force required to puncture a soft material is critical in many fields like medical technology, food processing, and manufacturing. However, such a prediction strongly depends on our understanding of the complex nonlinear behavior of the material subject to deep indentation and complex failure mechanisms. Only recently we developed theories capable of correlating puncture force with material properties and needle geometry. However, such models are based on simplifications that seldom limit their applicability to real cases. One common assumption is the incompressibility of the cut material, albeit no material is truly incompressible. In this paper we propose a simple model that accounts for linearly elastic compressibility, and its interplay with toughness, stiffness, and elastic strain-stiffening. Confirming previous theories and experiments, materials having high-toughness and low-modulus exhibit the highest puncture resistance at a given needle radius. Surprisingly, in these conditions, we observe that incompressible materials exhibit the lowest puncture resistance, where volumetric compressibility can create an additional (strain) energy barrier to puncture. Our model provides a valuable tool to assess the puncture resistance of soft compressible materials and suggests new design strategies for sharp needles and puncture-resistant materials.",2304.13838v1 2008-05-23,Non-hysteretic branches inside the hysteresis loop in VO2 films for focal plane array imaging bolometers,"In the resistive phase transition in VO2, temperature excursions from points on the major hysteresis loop produce minor loops. We have found that for sufficiently small excursions these minor loops degenerate into single-valued, non-hysteretic branches (NHBs) having essentially the same or even higher temperature coefficient of resistance (TCR) as the semiconducting phase at room temperature. We explain this behavior and discuss the opportunities it presents for infrared imaging technology based on resistive microbolometers. It is possible to choose a NHB with 100 to 1000 times smaller resistivity than in a pure semiconducting phase, thus providing a microbolometer with low tunable resistivity and high TCR.",0805.3566v1 2021-05-26,Investigation of Forming Free Bipolar Resistive Switching Characteristics in Al/Mn3O4/FTO RRAM Device,"Bipolar resistive switching (BRS) phenomenon has been demonstrated in Mn3O4 using Al (Aluminum)/Mn3O4/FTO (Fluorine doped Tin Oxide) Resistive Random Access Memory (RRAM) device. The fabricated RRAM device shows good retention, non volatile behavior and forming free BRS. The Current-Voltage (I-V) characteristics and the temperature dependence of the resistance (R-T) measurements were used to explore conduction mechanisms and the thermal activation energy (Ea). The resistance ratio of high resistance state (HRS) to low resistance state (LRS) is ~102. The fabricated RRAM device shows different conduction mechanisms in LRS and HRS state such as ohmic conduction and space charge limited conduction (SCLC). The rupture and formation of conducting filaments (CF) of oxygen vacancies take place by changing the polarity of external voltage, which may be responsible for resistive switching characteristics in the fabricated RRAM device. This fabricated RRAM device is suitable for application in future high density non-volatile memory (NVM) RRAM devices.",2105.12390v1 1998-08-18,Resistivity saturation revisited: results from a dynamical mean field theory,"We use the dynamical mean field method to study the high-temperature resistivity of electrons strongly coupled to phonons. The results reproduce the qualtiative behavior of the temperature and disorder dependence of the resistivity of the 'A-15' materials, which is commonly described in terms of saturation, but imply that the resistivity does not saturate. Rather, a change in temperature dependence occurs when the scattering becomes strong enough to cause a breakdown of the Migdal approximation.",9808188v2 2018-07-13,A new type of RPC with very low resistive material,"There are several working groups that are currently working on high rate RPC's using different materials such as Si-based Ceramics, Low-resistive Glass, low-resistive bakelite etc. A new type of single gap RPC has been fabricated using very low-resistive carbon-loaded PTFE material to compete with all these other groups and materials. In terms of bulk resistivity, this material is the lowest and should in principle be able to work at the highest rates, provided the material can withstand working bias and radiation. The efficiency and noise rate of the RPC are measured with cosmic rays. The detail method of fabrication and first experimental results are presented.",1807.04984v1 2013-04-20,Electric-Field-Induced Resistive Switching in a Family of Mott Insulators : towards Non-Volatile Mott-RRAM Memories,"The fundamental building blocks of modern silicon-based microelectronics, such as double gate transistors in non-volatile Flash memories, are based on the control of electrical resistance by electrostatic charging. Flash memories could soon reach their miniaturization limits mostly because reliably keeping enough electrons in an always smaller cell size will become increasingly difficult . The control of electrical resistance at the nanometer scale therefore requires new concepts, and the ultimate resistance-change device is believed to exploit a purely electronic phase change such as the Mott insulator to insulator transition [2]. Here we show that application of short electric pulses allows to switch back and forth between an initial high-resistance insulating state (""0"" state) and a low-resistance ""metallic"" state (""1"" state) in the whole class of Mott Insulator compounds AM4X8 (A = Ga, Ge; M= V, Nb, Ta; X = S, Se). We found that electric fields as low as 2 kV/cm induce an electronic phase change in these compounds from a Mott insulating state to a metallic-like state. Our results suggest that this transition belongs to a new class of resistive switching and might be explained by recent theoretical works predicting that an insulator to metal transition can be achieved by a simple electric field in a Mott Insulator. This new type of resistive switching has potential to build up a new class of Resistive Random Access Memory (RRAM) with fast writing/erasing times (50 ns to 10 {\mu}s) and resistance ratios \Delta R/R of the order of 25% at room temperature.",1304.5607v1 2012-06-26,Measurement of electrical properties of electrode materials for the bakelite Resistive Plate Chambers,"Single gap (gas gap 2 mm) bakelite Resistive Plate Chamber (RPC) modules of various sizes from 10 cm \times 10 cm to 1 m \times 1 m have been fabricated, characterized and optimized for efficiency and time resolution. Thin layers of different grades of silicone compound are applied to the inner electrode surfaces to make them smooth and also to reduce the surface resistivity. In the silicone coated RPCs an efficiency > 90% and time resolution \sim 2 ns (FWHM) have been obtained for both the streamer and the avalanche mode of operation. Before fabrication of detectors the electrical properties such as bulk resistivity and surface resistivity of the electrode materials are measured carefully. Effectiveness of different silicone coating in modifying the surface resistivity was evaluated by an instrument developed for monitoring the I-V curve of a high resistive surface. The results indicate definite correlation of the detector efficiency for the atmospheric muons and the RPC noise rates with the surface resistivity and its variation with the applied bias voltage. It was also found that the surface resistivity varies for different grades of silicone material applied as coating, and the results are found to be consistent with the detector efficiency and noise rate measurements done with these RPCs.",1206.5894v1 2015-09-21,Resistive Switching in Nanodevices,"Passing current at given threshold voltages through a metal/insulator/metal sandwich structure device may change its resistive state. Such resistive switching is unique to nanoscale devices, but its underlying physical mechanism remains unknown. We show that the different resistive states are due to different spontaneously charged states, characterized by different `band bending' solutions of Poisson's equation. For an insulator with mainly donor type defects, the low-resistivity state is characterized by a negatively charged insulator due to convex band bending, and the high-resistivity state by a positively charged insulator due to concave band bending; vice versa for insulators with mainly acceptor type defects. These multiple solutions coexist only for nanoscale devices and for bias voltages limited by the switching threshold values, where the system charge spontaneously changes and the system switches to another resistive state. We outline the general principles how this functionality depends on material properties and defect abundance of the insulator `storage medium', and propose a new magnetic memristor device with increased storage capacity.",1509.06169v1 2018-06-30,Nanoscale compositional evolution in complex oxide based resistive memories,"Functional oxides based resistive memories are recognized as potential candidate for the next-generation high density data storage and neuromorphic applications. Fundamental understanding of the compositional changes in the functional oxides is required to tune the resistive switching characteristics for enhanced memory performance. Herein, we present the micro/nano-structural and compositional changes induced in a resistive oxide memory during resistive switching. Oxygen deficient amorphous chromium doped strontium titanate (Cr:$a$-SrTiO$_{3-x}$) based resistance change memories are fabricated in a Ti/Cr:$a$-SrTiO$_{3-x}$ heterostructure and subjected to different biasing conditions to set memory states. Transmission electron microscope based cross-sectional analyses of the memory devices in different memory states shows that the micro/nano-structural changes in amorphous complex oxide and associated redox processes define the resistive switching behavior. These experimental results provide insights and supporting material for Ref. [1].",1807.00185v1 2018-06-04,"Atomistic Study of the Electronic Contact Resistivity Between the Half-Heusler Alloys (HfCoSb, HfZrCoSb, HfZrNiSn) and the Metal Ag","Half-Heusler(HH) alloys have shown promising thermoelectric properties in the medium and high temperature range. To harness these material properties for thermoelectric applications, it is important to realize electrical contacts with low electrical contact resistivity. However, little is known about the detailed structural and electronic properties of such contacts, and the expected values of contact resistivity. Here, we employ atomistic ab initio calculations to study electrical contacts in a subclass of HH alloys consisting of the compounds HfCoSb, HfZrCoSb, and HfZrNiSn. By using Ag as a prototypical metal, we show that the termination of the HH material critically determines the presence or absence of strong deformations at the interface. Our study includes contacts to doped materials, and the results indicate that the p-type materials generally form ohmic contacts while the n-type materials have a small Schottky barrier. We calculate the temperature dependence of the contact resistivity in the low to medium temperature range and provide quantitative values that set lower limits for these systems.",1806.01375v1 2009-01-28,Carbon Based Resistive Memory,"We propose carbon as new resistive memory material for non-volatile memories and compare three allotropes of carbon, namely carbon nanotubes, graphene-like conductive carbon and insulating carbon for their possible application as resistance-change material in high density non-volatile memories. Repetitive high-speed switching and the potential for multi-level programming have been successfully demonstrated.",0901.4439v1 2016-01-31,Josephson-like Colossal Resistive Switching in Nanocrystalline Y-Ba-Cu-O at Room Temperature,"In this paper, we present data for two nanocrystalline YBa2Cu3O7-x (YBCO) samples which both exhibit Josephson-like Colossal Resistive Switching (JCRS) in voltage-current (V-I) traces from 4.2 K up to room temperature, in magnetic fields up to 8 T. We report Josephson-like hysteresis for both positive and negative current that has not been observed before in colossal resistive switching materials. Non-zero resistance was measured in transport measurements at all temperatures. At low temperatures (< 90 K), we also observed the usual properties for YBCO including weak superconducting and paramagnetic behavior, measured using ac susceptibility and magnetization measurements. The resistivity of these nanocrystalline samples is 3 orders of magnitude higher than standard polycrystalline materials at 300 K and the temperature dependence semiconductor-like. We cannot rule out the possibility that these materials contain a superconducting component responsible for the JCRS behavior at room temperature.",1602.00271v3 2013-08-28,First studies with the Resistive-Plate WELL gaseous multiplier,"We present the results of first studies of the Resistive Plate WELL (RPWELL): a single-faced THGEM coupled to a copper anode via a resistive layer of high bulk resistivity. We explored various materials of different bulk resistivity (10^9 - 10^12 Ohm cm) and thickness (0.4 - 4 mm). Our most successful prototype, with a 0.6 mm resistive plate of ~10^9 Ohm cm, achieved gains of up to 10^5 with 8 keV x-ray in Ne/5%CH4; a minor 30% gain drop occurred with a rate increase from 10 to 10^4 Hz/mm^2. The detector displayed a full ""discharge-free"" operation--even when exposed to high primary ionization events. We present the RPWELL detector concept and compare its performance to that of other previously explored THGEM configurations--in terms of gain, its curves, dependence on rate, and the response to high ionization. The robust Resistive Plate WELL concept is a step forward in the Micro-Pattern Gas-Detector family, with numerous potential applications.",1308.6152v1 2021-02-07,Quantum Conductors Formation and Resistive Switching Memory Effects in Zirconia Nanotubes,"The development prospects of memristive elements for non-volatile memory with use of the metal-dielectric-metal sandwich structures with a thin oxide layer are due to the possibility of reliable forming the sustained functional states with quantized resistance. In the paper we study the properties of fabricated memristors based on the non-stoichiometric $ZrO_2$ nanotubes in different resistive switching modes. Anodic oxidation of the $Zr$ foil has been used to synthesize a zirconia layer of $1.7$ $\mu$$m$ thickness, consisting of an ordered array of vertically oriented nanotubes with outer diameter of 75 nm. $Zr/ZrO_2/Au$ sandwich structures have been fabricated by mask magnetron deposition. The effects of resistive switching in the $Zr/ZrO_2/Au$ memristors in unipolar and bipolar modes have been investigated. The resistance ratios $\geq3\cdot10^4$ between high-resistance (HRS) and low-resistance (LRS) states have been evaluated. It has been founded the conductivity of LRS is quantized in a wide range with minimum value of $0.5G_0=38.74$ $\mu$$S$ due to the formation of quantum conductors based on oxygen vacancies ($V_O$). Resistive switching mechanisms of $Zr/ZrO_2/Au$ memristors with allowing for migration of $V_O$ in an applied electric field have been proposed. It has been shown that the ohmic type and space charge limited conductivities are realized in the LRS and HRS, correspondingly. We present the results which can be used for development of effective memristors based on functional $Zr/ZrO_2/Au$ nanolayered structure with multiple resistive states and high resistance ratio.",2102.03764v1 2004-07-16,Negative Differential Resistivity and Positive Temperature Coefficient of Resistivity effect in the diffusion limited current of ferroelectric thin film capacitors,"We present a model for the leakage current in ferroelectric thin- film capacitors which explains two of the observed phenomena that have escaped satisfactory explanation, i.e. the occurrence of either a plateau or negative differential resistivity at low voltages, and the observation of a Positive Temperature Coefficient of Resistivity (PTCR) effect in certain samples in the high-voltage regime. The leakage current is modelled by considering a diffusion-limited current process, which in the high-voltage regime recovers the diffusion-limited Schottky relationship of Simmons already shown to be applicable in these systems.",0407428v1 2015-05-18,Nonpolar resistive memory switching with all four possible resistive switching modes in amorphous ternary rare earth LaHoO3 thin films,"We studied the resistive memory switching in pulsed laser deposited amorphous LaHoO3 (LHO) thin films for non-volatile resistive random access memory (RRAM) applications. Nonpolar resistive switching (RS) was achieved in PtLHOPt memory cells with all four possible RS modes ( positive unipolar, positive bipolar, negative unipolar, and negative bipolar) having high RON and ROFF ratios (in the range of 104 to 105) and non-overlapping switching voltages (set voltage, VON 3.6 to 4.2 V and reset voltage, VOFF 1.3 to 1.6 V) with a small variation of about 5 to 8 percent. X ray photoelectron spectroscopic studies together with temperature dependent switching characteristics revealed the formation of metallic holmium (Ho) and oxygen vacancies (VO) constituted conductive nanofilaments (CNFs) in the low resistance state (LRS). Detailed analysis of current versus voltage characteristics further corroborated the formation of CNFs based on metal like (Ohmic) conduction in LRS. Simmons Schottky emission was found to be the dominant charge transport mechanism in the high resistance state.",1505.04690v1 2019-07-23,Electron transport in high-entropy alloys: Al$_{x}$CrFeCoNi as a case study,"The high-entropy alloys Al$_{x}$CrFeCoNi exist over a broad range of Al concentrations ($0 < x < 2$). With increasing Al content their structure is changed from the fcc to bcc phase. We investigate the effect of such structural changes on transport properties including the residual resistivity and the anomalous Hall resistivity. We have performed a detailed comparison of the first-principles simulations with available experimental data. We show that the calculated residual resistivities for all studied alloy compositions are in a fair agreement with available experimental data as concerns both the resistivity values and concentration trends. We emphasize that a good agreement with experiment was obtained also for the anomalous Hall resistivity. We have completed study by estimation of the anisotropic magnetoresistance, spin-disorder resistivity, and Gilbert damping. The obtained results prove that the main scattering mechanism is due to the intrinsic chemical disorder whereas the effect of spin polarization on the residual resistivity is appreciably weaker.",1907.09731v1 2018-04-14,Investigating the Composite/Metal Interface and its Influence on the Electrical Resistance Measurement,"The advantages introduced by carbon fiber reinforced polymer (CFRP) composites has made them an appropriate choice in many applications and an ideal replacement for conventional materials. The benefits using CFRP composites are due to their lightweight, high stiffness, as well as corrosion resistance. For this reason, there is a fast growing trend in using CFRP composites for aircraft and wind turbine structural applications. The replacement of the conventional aerospace-grade metal alloys (aluminum, titanium, magnesium, etc.) with CFRP composites results in new challenges. For example, an aircraft during flight is prone to be struck by lightning. To withstand the injection of such massive amount of energy, adequate electrical properties, mainly electrical conductivity, is required. In fact, electrical conductance (or its reciprocal, resistance) is a critical parameter representing any material change and it can be considered an index for health monitoring. In this paper, AS4/8552 carbon/epoxy laminated composites were injected with two types of electrical currents, impulse current and direct current. The change in measured electrical resistance was recorded. A significant resistance drop occurred after electrical current injections. Furthermore, four-point flexural tests were performed on these composites to correlate an electrical resistance change with a potential flexural property change. There was no clear trend between a resistance change and flexural strength/modulus change of the test coupons, regardless of current injection. However, it was observed that the injection of the current affects the contact resistance such that its resistance decreases.",1804.06246v1 2018-08-09,Underlying burning resistant mechanisms for titanium alloy,"The ""titanium fire"" as produced during high pressure and friction is the major failure scenario for aero-engines. To alleviate this issue, Ti-V-Cr and Ti-Cu-Al series burn resistant titanium alloys have been developed. However, which burn resistant alloy exhibit better property with reasonable cost needs to be evaluated. This work unveils the burning mechanisms of these alloys and discusses whether burn resistance of Cr and V can be replaced by Cu, on which thorough exploration is lacking. Two representative burn resistant alloys are considered, including Ti14(Ti-13Cu-1Al-0.2Si) and Ti40(Ti-25V-15Cr-0.2Si)alloys. Compared with the commercial non-burn resistant titanium alloy, i.e., TC4(Ti-6Al-4V)alloy, it has been found that both Ti14 and Ti40 alloys form ""protective"" shields during the burning process. Specifically, for Ti14 alloy, a clear Cu-rich layer is formed at the interface between burning product zone and heat affected zone, which consumes oxygen by producing Cu-O compounds and impedes the reaction with Ti-matrix. This work has established a fundamental understanding of burning resistant mechanisms for titanium alloys. Importantly, it is found that Cu could endow titanium alloys with similar burn resistant capability as that of V or Cr, which opens a cost-effective avenue to design burn resistant titanium alloys.",1808.02976v1 2005-10-03,Buffer-Enhanced Electrical-Pulse-Induced-Resistive Memory Effect in Thin Film Perovskites,"A multilayer perovskite thin film resistive memory device has been developed comprised of: a Pr0.7Ca0.3MnO3 (PCMO) perovskite oxide epitaxial layer on a YBCO bottom thin film electrode; a thin yttria stabilized zirconia (YSZ) buffer layer grown on the PCMO layer, and a gold thin film top electrode. The multi-layer thin film lattice structure has been characterized by XRD and TEM analyses showing a high quality heterostructure. I-AFM analysis indicated nano granular conductivity distributed uniformly throughout the PCMO film surface. With the addition of the YSZ buffer layer, the pulse voltage needed to switch the device is significantly reduced and the resistance-switching ratio is increased compared to a non-buffered resistance memory device, which is very important for the device fabrication. The magnetic field effect on the multilayer structure resistance at various temperatures shows CMR behavior for both high and low resistance states implying a bulk material component to the switch behavior.",0510060v1 2020-04-24,Solution-processed silver sulphide nanocrystal film for resistive switching memories,"Resistive switching memories allow electrical control of the conductivity of a material, by inducing a high resistance (OFF) or a low resistance (ON) state, using electrochemical and ion transport processes. As alternative to high temperature and vacuum-based physical sulphurization methods of silver (Ag), here we propose, as resistive switching medium, a layer built from colloidal Ag$_{2-x}$S nanocrystals -compatible with solution-processed approaches. The effect of the electrode size (from macro- to micro-scale), composition (Ag, Ti and Pt) and geometry on the device performance together with the electrochemical mechanisms involved are evaluated. We achieved an optimized Ag/Ti bowtie proof-of-concept configuration by e-beam lithography, which fulfils the general requirements for ReRAM devices in terms of low power consumption and reliable $I_{ON}/I_{OFF}$ ratio. This configuration demonstrates reproducible switching between ON and OFF states with data endurance of at least 20 cycles; and an $I_{ON}/I_{OFF}$ ratio up to 10$^3$ at low power consumption (0.1V readout), which outperforms previous results in literature for devices with resistive layers fabricated from silver chalcogenide nanoparticles.",2004.11875v1 2005-12-22,Measurement of Local Reactive and Resistive Photoresponse of a Superconducting Microwave Device,"We propose and demonstrate a spatial partition method for the high-frequency photo-response of superconducting devices correlated with inductive and resistive changes in microwave impedance. Using a laser scanning microscope, we show that resistive losses are mainly produced by local defects at microstrip edges and by intergrain weak links in the high-temperature superconducting material. These defects initiate nonlinear high-frequency response due to overcritical current densities and entry of vortices.",0512572v1 2002-10-28,Nanometer-Scale Metallic Grains Connected with Atomic-Scale Conductors,"We describe a technique for connecting a nanometer-scale gold grain to leads by atomic-scale gold point contacts. These devices differ from previous metallic quantum dots in that the conducting channels are relatively well-transmitting. We investigate the dependence of the Coulomb blockade on contact resistance. The high-resistance devices display Coulomb blockade and the low-resistance devices display a zero-bias conductance dip, both in quantitative agreement with theory. We find that in the intermediate regime, where the sample resistance is close to $h/e^2$, the I-V curve displays a Coulomb staircase with symmetric contact capacitances.",0210620v1 2004-08-05,Influence of Grain size on the Electrical Properties of ${\rm Sb_2Te_3}$ Polycrystalline Films,"Resistance of vacuum deposited ${\rm Sb_2Te_3}$ films of thickness between 100-500nm has been measured in vacuum. It is found that the resistance of the polycrystalline films strongly depends on the grain size and inter-granular voids. The charge carrier are shown to cross this high resistivity inter- granular void by ohmic conduction. The barrier height as well as temperature coefficient of resistance are also shown to depend on the grain size and inter- grain voids.",0408116v1 2008-05-03,Resistance Quenching in Graphene Interconnects,"We investigated experimentally the high-temperature electrical resistance of graphene interconnects. The test structures were fabricated using the focused ion beam from the single and bi-layer graphene produced by mechanical exfoliation. It was found that as temperature increases from 300 to 500K the resistance of the single- and bi-layer graphene interconnects drops down by 30% and 70%, respectively. The quenching and temperature dependence of the resistance were explained by the thermal generation of the electron-hole pairs and acoustic phonon scattering. The obtained results are important for the proposed applications of graphene as interconnects in integrated circuits.",0805.0334v1 2008-05-12,Negative differential resistance and pulsed current induced multi-level resistivity switching in charge ordered and disordered manganites,"We have investigated direct and pulsed current induced electroresistance in two manganites with different electronic and magnetic ground states: charge-orbital ordered 50 % Ca doped NdMnO3 and 50 % Mn doped LaNiO3. It has been shown that negative differential resistance observed at high current density in these compounds is related to Joule heating. However, bi-level and multi-level resistivity switching induced by variations in pulse width and pulse period at low current density can not be attributable to Joule heating alone. We discuss possible origins.",0805.1643v1 2012-07-13,Enhanced Resolution of Poly-(Methyl Methacrylate) Electron Resist by Thermal Processing,"Granular nanostructure of electron beam resist had limited the ultimate resolution of electron beam lithography. We report a thermal process to achieve a uniform and homogeneous amorphous thin film of poly methyl methacrylate electron resist. This thermal process consists of a short time-high temperature backing process in addition to precisely optimized development process conditions. Using this novel process, we patterned arrays of holes in a metal film with diameter smaller than 5nm. In addition, line edge roughness and surface roughness of the resist reduced to 1nm and 100pm respectively.",1207.3183v1 2016-11-12,Anomalous resistivity upturn in epitaxial L21-Co2MnAl films,"We report the controllable growth and the intriguing transport behavior of high-spin-polarization epitaxial L21-Co2MnAl films, which exhibit a low-temperature (T) resistivity upturn with pronounced T1/2 dependence, close relevance to structural disorder, and robust independence of magnetic fields. The resistivity upturn turns out to be qualitatively contradictory to weak localization, particle-particle channel electron-electron interaction (EEI), and orbital two-channel Kondo effect, leaving a three-dimensional particle-hole channel EEI the most likely physical source. Our result highlights a considerable tunability of the structural and electronic disorder of magnetic films by varying growth temperature, affording unprecedented insights into the spin polarization and the resistivity upturn.",1611.04013v2 2011-04-06,Temperature dependence of contact resistance of Au-Ti-Pd2Si-n+-Si ohmic contacts,"We investigated temperature dependence of contact resistance of an Au-Ti-Pd2Si ohmic contact to heavily doped n+-Si. The contact resistance increases with temperature owing to conduction through the metal shunts. In this case, the limiting process is diffusion input of electrons to the metal shunts. The proposed mechanism of contact resistance formation seems to realize also in the case of wide-gap semiconductors with high concentration of surface states and dislocation density in the contact.",1104.1030v1 2021-04-25,Electrical resistivity in 2d Kondo lattice systems,"I extend the calculations represented in \cite{konav} regarding the resistivity in Kondo lattice materials from $3d$ syatem to $2d$ systems. In the present work I consider a 2d system, and memory function is computed. However, results found in 2d case are different from 3d system . I find that in $2d$ in low temperature regime($ k_{B}T\ll \mu_d$) resistivity shows power law($\frac{1}{T}$) behaviour and in the high temeprature regime($ k_{B}T\gg\mu_d$) resistivity varies linearly with temperature. In $3d$ these behaviours are as $\frac{1}{T}$ and as $T^{\frac{3}{2}}$ respectively.",2104.12129v1 2008-01-22,Abnormal Resistance Switching Behaviors of NiO Thin Films: Possible Occurrence of Simultaneous Formation and Rupture of Conducting Channels,"We report the detailed current-voltage (I-V) characteristics of resistance switching in NiO thin films. In unipolar resistance switching, it is commonly believed that conducting filaments will rupture when NiO changes from a low resistance to a high resistance state. However, we found that this resistance switching can sometimes show abnormal behavior during voltage- and current-driven I-V measurements. We used the random circuit breaker network model to explain how abnormal switching behaviors could occur. We found that this resistance change can occur via a series of avalanche processes, where conducting filaments could be formed as well as ruptured.",0801.3323v1 2009-08-12,Large 1/f noise of unipolar resistance switching and its percolating nature,"We investigated the 1/f noise of Pt/NiO/Pt capacitors that show unipolar resistance switching. When they were switched from the low to high resistance states, the power spectral density of the voltage fluctuation was increased by approximately five orders of magnitude. At 100 K, the relative resistance fluctuation, SR/R2, in the low resistance state displayed a power law dependence on the resistance R with exponent w = 1.6. This behavior can be explained by percolation theory; however, at higher temperatures or near the switching voltage, SR/R2 becomes enhanced further. This large 1/f noise can be therefore an important problem in the development of resistance random access memory devices.",0908.1606v1 2017-04-11,Scalability of Voltage-Controlled Filamentary and Nanometallic Resistance Memories,"Much effort has been devoted to device and materials engineering to realize nanoscale resistance random access memory (RRAM) for practical applications, but there still lacks a rational physical basis to be relied on to design scalable devices spanning many length scales. In particular, the critical switching criterion is not clear for RRAM devices in which resistance changes are limited to localized nanoscale filaments that experience concentrated heat, electric current and field. Here, we demonstrate voltage-controlled resistance switching for macro and nano devices in both filamentary RRAM and nanometallic RRAM, the latter switches uniformly and does not require forming. As a result, using a constant current density as the compliance, we have achieved area-scalability for the low resistance state of the filamentary RRAM, and for both the low and high resistance states of the nanometallic RRAM. This finding will help design area-scalable RRAM at the nanoscale.",1704.03415v1 2021-10-07,A Modern-day Alchemy: Double Glow Plasma Surface Metallurgy Technology,"In the long history of science and technology development, one goal is to diffuse solid alloy elements into the surface of steel materials to form surface alloys with excellent physical and chemical properties. On the basis of plasma nitriding technology, double glow plasma surface metallurgy technology has answered this challenge. This technology, which seems to be a modern-day alchemy, can use any element in the periodic table of chemical elements, including solid metal elements and their combinations, to form many types of surface alloyed layers with high hardness, wear resistance, corrosion resistance and high temperature oxidation resistance on various metal materials. For examples, nickel base alloys, stainless steels and high speed steels are formed on the surfaces of ordinary carbon steels; and high hardness, wear resistance and high temperature oxidation resistance alloy are formed on the surface of titanium alloy.This article briefly introduces the formation and principle of double glow plasma surface metallurgy technology, and summarizes the experimental results and industry application. The significance and development prospect of this technology are discussed.",2110.03236v1 2019-09-15,Large Resistivity Reduction in Mixed-Valent CsAuBr$_3$ Under Pressure,"We report on high-pressure $p \leq 45$ GPa resistivity measurements on the perovskite-related mixed-valent compound CsAuBr$_3$. The compounds high-pressure resistivity can be classified into three regions: For low pressures ($p < 10$ GPa) an insulator to metal transition is observed; between $p= 10$ GPa and 14 GPa the room temperature resistivity goes through a minimum and increases again; above $p = 14$ GPa a semiconducting state is observed. From this pressure up to the highest pressure of $p = 45$ GPa reached in this experiment, the room-temperature resistivity remains nearly constant. We find an extremely large resistivity reduction between ambient pressure and 10 GPa by more than 6 orders of magnitude. This decrease is among the largest reported changes in the resistivity for this narrow pressure regime. We show - by an analysis of the electronic band structure evolution of this material - that the large change in resistivity under pressure in not caused by a crossing of the bands at the Fermi level. We find that it instead stems from two bands that are pinned at the Fermi level and that are moving towards one another as a consequence of the mixed-valent to single-valent transition. This mechanism appears to be especially effective for the rapid buildup of the density of states at the Fermi level.",1909.06874v1 2023-02-25,"Peculiarities of electron transport and resistive switching in point contacts on TiSe2, TiSeS and CuxTiSe2","TiSe2 has received much attention among the transition metals chalcogenides because of its thrilling physical properties concerning atypical resistivity behavior, emerging of charge density wave (CDW) state, induced superconductivity etc. Here, we report discovery of new feature of TiSe2, namely, observation of resistive switching in voltage biased point contacts (PCs) based on TiSe2 and its derivatives doped by S and Cu (TiSeS, CuxTiSe2). The switching is taking place between a low resistive mainly metallic-type state and a high resistive semiconducting-type state by applying bias voltage (usually below 0.5V), while reverse switching takes place by applying voltage of opposite polarity (usually below 0.5V). The difference in resistance between these two states can reach up to two orders of magnitude at the room temperature. The origin of the effect can be attributed to the variation of stoichiometry in PC core due to drift/displacement of Se/Ti vacancies under high electric field. Additionally, we demonstrated, that heating takes place in PC core, which can facilitate the electric field induced effect. At the same time, we did not found any evidence for CDW spectral features in our PC spectra for TiSe2. The observed resistive switching allows to propose TiSe2 and their derivatives as the promising materials, e.g., for non-volatile resistive random access memory (ReRAM) engineering.",2302.13085v1 2021-04-21,A First-Principles-Based Approach to The High-Throughput Screening of Corrosion-Resistant High Entropy Alloys,"The design of corrosion-resistant high entropy alloys (CR-HEAs) is challenging due to the alloys' virtually astrological composition space. To facilitate this, efficient and reliable high-throughput exploratory approaches are needed. Toward this end, the current work reports a first-principles-based approach exploiting the correlations between work function, surface energy, and corrosion resistance (i.e., work function and surface energy are, by definitions, proportional and inversely proportional to an alloy's inherent corrosion resistance, respectively). Two Bayesian CALPHAD models (or databases) of work function and surface energy of FCC Co-Cr-Fe-Mn-Mo-Ni are assessed using discrete surface energies and work functions derived by density-functional theory (DFT) calculations. The models are then used to rank different Co-Cr-Fe-Mn-Mo-Ni alloy compositions. It is observed that the ranked alloys possess chemical traits similar to previously studied corrosion-resistance alloys, suggesting that the proposed approach can be used to reliably screen HEAs with potentially good inherent corrosion resistance.",2104.10590v1 2023-04-02,Percolation-induced resistivity drop in cold-pressed LuH2,"The stoichiometric bulk LuH2 is a paramagnetic metal with high electrical conductivity comparable to simple metals. Here we show that the resistivity of cold-pressed (CP) LuH2 samples varies sensitively upon modifying the grain size or surface conditions via the grinding process, i.e., the CP pellets made of commercially purchased LuH2 powder remain metallic but exhibit thousands of times higher resistivity, while additional grinding of LuH2 powders in air further enhances the resistivity and even results in weakly localized behaviors. For these CP samples, interestingly, we can occasionally observe abrupt resistivity drops at high temperatures, which also show dependences on magnetic fields and electrical current. Measurements of variable-temperature XRD, magnetic susceptibility, and specific heat exclude the possibilities of structural, magnetic, and superconducting transitions for the observed resistivity drops. Instead, we tentatively attribute these above observations to the presence of insulating layers on the grain surface due to the modification of hydrogen stoichiometry or the pollution by oxygen/nitrogen. Percolation of the metallic grains through the insulating surfaces can explain the sudden drop in resistivity. The present results thus call for caution in asserting the resistivity drops as superconductivity and invalidate the background subtraction in analyzing the resistivity data.",2304.00558v1 2017-07-28,High-temperature quantum oscillations of the Hall resistance in bulk Bi$_2$Se$_3$,"Helically spin-polarized Dirac fermions (HSDF) in protected topological surface states (TSS) are of high interest as a new state of quantum matter. In three-dimensional (3D) materials with TSS, electronic bulk states often mask the transport properties of HSDF. Recently, the high-field Hall resistance and low-field magnetoresistance indicate that the TSS may coexist with a layered two-dimensional electronic system (2DES). Here, we demonstrate quantum oscillations of the Hall resistance at temperatures up to 50 K in bulk Bi$_2$Se$_3$ with a high electron density $n$ of about $2\!\cdot\!10^{19}$ cm$^{-3}$. From the angular and temperature dependence of the Hall resistance and the Shubnikov-de Haas oscillations we identify 3D and 2D contributions to transport. Angular resolved photoemission spectroscopy proves the existence of TSS. We present a model for Bi$_2$Se$_3$ and suggest that the coexistence of TSS and 2D layered transport stabilizes the quantum oscillations of the Hall resistance.",1707.09181v1 2005-11-15,Unconventional Hall effect in oriented Ca$_3$Co$_4$O$_9$ thin films,"Transport properties of the good thermoelectric misfit oxide Ca$_3$Co$_4$O$_9$ are examined. In-plane resistivity and Hall resistance measurements were made on epitaxial thin films which were grown on {\it c}-cut sapphire substrates using the pulsed laser deposition technique. Interpretation of the in-plane transport experiments relates the substrate-induced strain in the resulting film to single crystals under very high pressure ($\sim$ 5.5 GPa) consistent with a key role of strong electronic correlation. They are confirmed by the measured high temperature maxima in both resistivity and Hall resistance. While hole-like charge carriers are inferred from the Hall effect measurements over the whole investigated temperature range, the Hall resistance reveals a non monotonic behavior at low temperatures that could be interpreted with an anomalous contribution. The resulting unconventional temperature dependence of the Hall resistance seems thus to combine high temperature strongly correlated features above 340 K and anomalous Hall effect at low temperature, below 100 K.",0511374v1 2013-10-21,Micro Pixel Chamber with resistive electrodes for spark reduction,"The Micro Pixel Chamber (mu-PIC) using resistive electrodes has been developed and tested. The surface cathodes are made from resistive material, by which the electrical field is reduced when large current is flowed. Two-dimensional readouts are achieved by anodes and pickup electrodes, on which signals are induced. High gas gain (> 60000) was measured using 55Fe (5.9 keV) source, and very intensive spark reduction was attained under fast neutron. The spark rate of resistive mu-PIC was only 10^-4 times less than that of conventional mu-PIC at the gain of 10^4. With these developments, a new MPGD with no floating structure is achieved, with enough properties of both high gain and good stability to detect MIP particles. In addition, mu-PIC can be operated with no HV applied on anodes by using resistive cathodes. Neither AC coupling capacitors nor HV pull up resisters are needed for any anode electrode. Signal readout is drastically simplified by that configuration.",1310.5550v1 2023-11-28,Quantifying the contribution of material and junction resistances in nano-networks,"Networks of nanowires and nanosheets are important for many applications in printed electronics. However, the network conductivity and mobility are usually limited by the inter-particle junction resistance, a property that is challenging to minimise because it is difficult to measure. Here, we develop a simple model for conduction in networks of 1D or 2D nanomaterials, which allows us to extract junction and nanoparticle resistances from particle-size-dependent D.C. resistivity data of conducting and semiconducting materials. We find junction resistances in porous networks to scale with nanoparticle resistivity and vary from 5 Ohm for silver nanosheets to 25 GOhm for WS2 nanosheets. Moreover, our model allows junction and nanoparticle resistances to be extracted from A.C. impedance spectra of semiconducting networks. Impedance data links the high mobility (~7 cm2/Vs) of aligned networks of electrochemically exfoliated MoS2 nanosheets to low junction resistances of ~670 kOhm. Temperature-dependent impedance measurements allow us to quantitatively differentiate intra-nanosheet phonon-limited band-like transport from inter-nanosheet hopping for the first time.",2311.16740v1 2016-02-04,"Low-Resistance 2D/2D Ohmic Contacts: A Universal Approach to High-Performance WSe2, MoS2, and MoSe2 Transistors","We report a new strategy for fabricating 2D/2D low-resistance ohmic contacts for a variety of transition metal dichalcogenides (TMDs) using van der Waals assembly of substitutionally doped TMDs as drain/source contacts and TMDs with no intentional doping as channel materials. We demonstrate that few-layer WSe2 field-effect transistors (FETs) with 2D/2D contacts exhibit low contact resistances of ~ 0.3 k ohm.um, high on/off ratios up to > 109, and high drive currents exceeding 320 uA um-1. These favorable characteristics are combined with a two-terminal field-effect hole mobility ~ 2x102 cm2 V-1 s-1 at room temperature, which increases to >2x103 cm2 V-1 s-1 at cryogenic temperatures. We observe a similar performance also in MoS2 and MoSe2 FETs with 2D/2D drain and source contacts. The 2D/2D low-resistance ohmic contacts presented here represent a new device paradigm that overcomes a significant bottleneck in the performance of TMDs and a wide variety of other 2D materials as the channel materials in post-silicon electronics.",1602.01790v1 2013-12-30,Deviations from Matthiessen rule and resistivity saturation effects in Gd and Fe,"According to earlier first-principles calculations, the spin-disorder contribution to the resistivity of rare-earth metals in the paramagnetic state is strongly underestimated if Matthiessen's rule is assumed to hold. To understand this discrepancy, the resistivity of paramagnetic Fe and Gd is evaluated by taking into account both spin and phonon disorder. Calculations are performed using the supercell approach within the linear muffin-tin orbital method. Phonon disorder is modeled by introducing random displacements of the atomic nuclei, and the results are compared with the case of fictitious Anderson disorder. In both cases the resistivity shows a nonlinear dependence on the square of the disorder potential, which is interpreted as a resistivity saturation effect. This effect is much stronger in Gd than in Fe. The non-linearity makes the phonon and spin-disorder contributions to the resistivity non-additive, and the standard procedure of extracting the spin-disorder resistivity by extrapolation from high temperatures becomes ambiguous. An ""apparent"" spin-disorder resistivity obtained through such extrapolation is in much better agreement with experiment compared to the results obtained by considering only spin disorder. By analyzing the spectral function of the paramagnetic Gd in the presence of Anderson disorder, the resistivity saturation is explained by the collapse of a large area of the Fermi surface due to the disorder-induced mixing between the electronic and hole sheets.",1312.7802v1 2016-11-08,Controlling friction in a manganite surface by resistive switching,"We report a significant change in friction of a $\rm La_{0.55}Ca_{0.45}MnO_3$ thin film measured as a function of the materials resistive state under ultrahigh vacuum conditions at room temperature by friction force microscopy. While friction is high in the insulating state, it clearly changes to lower values if the probed local region is switched to the conducting state via nanoscale resistance switching. Thus we demonstrate active control of friction without having to change the temperature or pressure. Upon switching back to an insulating state the friction increases again. The results are discussed in the framework of electronic friction effects and electrostatic interactions.",1611.02684v1 2019-10-05,Metamaterial insertions for resistive-wall beam-coupling impedance reduction,"Resistive-wall impedance usually constitutes a significant percentage of the total beamcoupling impedance budget of an accelerator. Reduction techniques often entail high electrical-conductivity coatings. This paper investigates the use of negative-permittivity or negative-permeability materials for sensibly reducing or theoretically nearly cancelling resistive-wall impedance. The proposed approach is developed by means of an equivalent transmission-line model. The effectiveness of such materials is benchmarked for the negative permeability case with experimental measurements in two frequency bandwidths. This first-stage study opens the possibility of considering metamaterials for impedance mitigation.",1910.02246v1 2020-07-07,Resistivity saturation in an electron-doped cuprate,"We report the observation of resistivity saturation in lightly doped ($x\sim 0.10)$ as-grown samples of the electron-doped cuprate La$_{2-x}$Ce$_x$CuO$_4$ (LCCO). The saturation occurs at resistivity values roughly consistent with the phenomenological Mott-Ioffe-Regel criterion once the low effective carrier density of these materials is included in the analysis. These results imply that, at least for light doping, the high-temperature metallic phase of these materials is not necessarily strange and may be understood as simply a low-density metal.",2007.03685v1 2015-06-24,Resonant tunneling in a quantum oxide superlattice,"Resonant tunnelling is a quantum mechanical process that has long been attracting both scientific and technological attention owing to its intriguing underlying physics and unique applications for high-speed electronics. The materials system exhibiting resonant tunnelling, however, has been largely limited to the conventional semiconductors, partially due to their excellent crystalline quality. Here we show that a deliberately designed transition metal oxide superlattice exhibits a resonant tunnelling behaviour with a clear negative differential resistance. The tunnelling occurred through an atomically thin, lanthanum {\delta}-doped SrTiO3 layer, and the negative differential resistance was realized on top of the bipolar resistance switching typically observed for perovskite oxide junctions. This combined process resulted in an extremely large resistance ratio (~10^5) between the high and low-resistance states. The unprecedentedly large control found in atomically thin {\delta}-doped oxide superlattices can open a door to novel oxide-based high-frequency logic devices.",1506.07583v1 2021-08-26,An investigation of high entropy alloy conductivity using first-principles calculations,"The Kubo-Greenwood equation, in combination with the first-principles Korringa-Kohn-Rostoker Coherent Potential Approximation (KKR-CPA) can be used to calculate the DC residual resistivity of random alloys at T = 0 K. We implemented this method in a multiple scattering theory based ab initio package, MuST, and applied it to the ab initio study of the residual resistivity of the high entropy alloy Al$_x$CoCrFeNi as a function of $x$. The calculated resistivities are compared with experimental data. We also predict the residual resistivity of refractory high entropy alloy MoNbTaV$_x$W. The calculated resistivity trends are also explained using theoretical arguments.",2108.11739v1 2024-01-27,Influence od the process parameters on the quality a efficiency of the resistance spot welding process of advanced high strength complex phase stells,"The effects of electrical characteristics of an inverter combined with main welding parameters on the resistance spot weldability of advanced high strength steels AHSS CP1000 is investigated.",2401.15457v1 2016-02-22,"The effect of Ta oxygen scavenger layer on HfO$_2$-based resistive switching behavior: thermodynamic stability, electronic structure, and low-bias transport","Reversible resistive switching between high-resistance and low-resistance states in metal-oxide-metal heterostructures makes them very interesting for applications in random access memories. While recent experimental work has shown that inserting a metallic ""oxygen scavenger layer"" between the positive electrode and oxide improves device performance, the fundamental understanding of how the scavenger layer modifies heterostructure properties is lacking. We use density functional theory to calculate thermodynamic properties and conductance of TiN/HfO$_2$/TiN heterostructures with and without Ta scavenger layer. First, we show that Ta insertion lowers the formation energy of low-resistance states. Second, while the Ta scavenger layer reduces the Schottky barrier height in the high-resistance state by modifying the interface charge at the oxide-electrode interface, the heterostructure maintains a high resistance ratio between high- and low-resistance states. Finally, we show that the low-bias conductance of device on-states becomes much less sensitive to the spatial distribution of oxygen removed from the HfO$_2$ in the presence of the Ta layer. By providing fundamental understanding of the observed improvements with scavenger layers, we open a path to engineer interfaces with oxygen scavenger layers to control and enhance device performance. In turn, this may enable the realization of a non-volatile low-power memory technology with concomitant reduction in energy consumption by consumer electronics and significant benefits to society.",1602.06793v1 2002-09-04,Electrical resistivity at large temperatures: Saturation and lack thereof,"Many transition metal compounds show saturation of the resistivity at high temperatures, T, while the alkali-doped fullerenes and the high-Tc cuprates are usually considered to show no saturation. We present a model of transition metal compounds, showing saturation, and a model of alkali-doped fullerenes, showing no saturation. To analyze the results we use the f-sum rule, which leads to an approximate upper limit for the resistivity at large T. For some systems and at low T, the resistivity increases so rapidly that this upper limit is approached for experimental T. The resistivity then saturates. For a model of transition metal compounds with weakly interacting electrons, the upper limit corresponds to a mean free path consistent with the Ioffe-Regel condition. For a model of the high Tc cuprates with strongly interacting electrons, however, the upper limit is much larger than the Ioffe-Regel condition suggests. Since this limit is not exceeded by experimental data, the data are consistent with saturation also for the cuprates. After ""saturation"" the resistivity usually grows slowly. For the alkali-doped fullerenes, ""saturation"" can be considered to have happened already for T=0, due to orientational disorder. For these systems, however, the resistivity grows so rapidly after ""saturation"" that this concept is meaningless. This is due to the small band width and to the coupling to the level energies of the important phonons.",0209099v1 2023-12-26,Corrosion-resistant aluminum alloy design through machine learning combined with high-throughput calculations,"Efficiently designing lightweight alloys with combined high corrosion resistance and mechanical properties remains an enduring topic in materials engineering. To this end, machine learning (ML) coupled ab-initio calculations is proposed within this study. Due to the inadequate accuracy of conventional stress-strain ML models caused by corrosion factors, a novel reinforcement self-learning ML algorithm (accuracy R2 >0.92) is developed. Then, a strategy that integrates ML models, calculated energetics and mechanical moduli is implemented to optimize the Al alloys. Next, this Computation Designed Corrosion-Resistant Al alloy is fabricated that verified the simulation. The performance (elongation reaches ~30%) is attributed to the H-captured Al-Sc-Cu phases (-1.44 eV H-1) and Cu-modified {\eta}/{\eta}' precipitation inside the grain boundaries (GBs). The developed Al-Mg-Zn-Cu interatomic potential (energy accuracy 6.50 meV atom-1) proves the cracking resistance of the GB region enhanced by Cu-modification. Conceptually, our strategy is of practical importance for designing new alloys exhibiting corrosion resistance and mechanical properties.",2312.15899v1 2001-03-01,Properties of Pt Schottky Type Contacts On High-Resistivity CdZnTe Detectors,"In this paper we present studies of the I-V characteristics of CdZnTe detectors with Pt contacts fabricated from high-resistivity single crystals grown by the high-pressure Brigman process. We have analyzed the experimental I-V curves using a model that approximates the CZT detector as a system consisting of a reversed Schottky contact in series with the bulk resistance. Least square fits to the experimental data yield 0.78-0.79 eV for the Pt-CZT Schottky barrier height, and <20 V for the voltage required to deplete a 2 mm thick CZT detector. We demonstrate that at high bias the thermionic current over the Schottky barrier, the height of which is reduced due to an interfacial layer between the contact and CZT material, controls the leakage current of the detectors. In many cases the dark current is not determined by the resistivity of the bulk material, but rather the properties of the contacts; namely by the interfacial layer between the contact and CZT material.",0103005v1 2010-01-27,"An anomalous butterfly-shaped magnetoresistance loop in an alloy, Tb4LuSi3","Magnetic-field (H) induced first-order magnetic transition and the assiciated electronic phase-separation phenomena are active topics of research in magnetism. Magnetoresistance (MR) is a key property to probe these phenomena and, in literature, a butterfly-shaped MR loop has been noted while cycling the field, with the envelope curve lying below the virgin curve in MR versus H plots of such materials. Here, we report an opposite behavior of MR loop for an alloy, Tb4LuSi3, at low temperatures (<<20 K) in the magnetically ordered state. Such an anomalous curve reveals unexpected domination of higher resistive high-field phase in electronic conduction, unlike in other materials where conducion is naturally by low-resistive high-field phase that follows first-order transition. The observed features reveal an unusual electronic phase separation, namely involving high-resistive high-field phase and low-resistive virgin phase.",1001.4942v1 2006-03-31,Clustering of vacancy defects in high-purity semi-insulating SiC,"Positron lifetime spectroscopy was used to study native vacancy defects in semi-insulating silicon carbide. The material is shown to contain (i) vacancy clusters consisting of 4--5 missing atoms and (ii) Si vacancy related negatively charged defects. The total open volume bound to the clusters anticorrelates with the electrical resistivity both in as-grown and annealed material. Our results suggest that Si vacancy related complexes compensate electrically the as-grown material, but migrate to increase the size of the clusters during annealing, leading to loss of resistivity.",0603849v3 2024-01-26,New perspectives of Hall effects from first-principles calculations,"The Hall effect has been a fascinating topic ever since its discovery, resulting in exploration of entire family of this intriguing phenomena. As the field of topology develops and novel materials emerge endlessly over the past few decades, researchers have been passionately debating the origins of various Hall effects. Differentiating between the ordinary Hall effect and extraordinary transport properties, like the anomalous Hall effect, can be quite challenging, especially in high-conductivity materials, including those with topological origins. In this study, we conduct a systematic and comprehensive analysis of Hall effects by combining the semiclassical Boltzmann transport theory with first principles calculations within the relaxation time approximation. We first highlight some striking similarities between the ordinary Hall effect and certain anomalous Hall effects, such as nonlinear dependency on magnetic field and potential sign reversal of the Hall resistivity. We then demonstrate that the Hall resistivity can be scaled with temperature and magnetic field as well, analogue to the Kohler's rule which scales the longitudinal resistivity under the relaxation time approximation. We then apply this Kohler's rule for Hall resistivity to two representative materials: ZrSiS and PtTe$_2$ with reasonable agreement with experimental measurement. Moreover, our methodology has been proven to be applicable to the planar Hall effects of bismuth, of perfect agreements with experimental observations. Our research on the scaling behavior of Hall resistivity addresses a significant gap in this field and provides a comprehensive framework for a deeper understanding of the Hall resistance family, and thus has potential to propel the field forward and spark further investigations into the fascinating world of Hall effects.",2401.15150v1 2012-04-12,Effect of crystallographic anisotropy on the resistance switching phenomenon in perovskites,"Resistance switching effects in metal/perovskite contacts based on epitaxial c-axis oriented Y-Ba-Cu-O (YBCO) thin films with different crystallographic orientations have been studied. Three types of Ag/YBCO junctions with the contact restricted to (i) c-axis direction, (ii) ab-plane direction, and (iii) both were designed and fabricated, and their current-voltage characteristics have been measured. The type (i) junctions exhibited conventional bipolar resistance switching behavior, whereas in other two types the low-resistance state was unsteady and their resistance quickly relaxed to the initial high-resistance state. Physical mechanism based on the oxygen diffusion scenario, explaining such behavior, is discussed.",1204.2598v1 2013-04-07,Characterization and simulation of resistive-MPGDs with resistive strip and layer topologies,"The use of resistive technologies to MPGD detectors is taking advantage for many new applications, including high rate and energetic particle flux scenarios. The recent use of these technologies in large area detectors makes necessary to understand and characterize the response of this type of detectors in order to optimize or constrain the parameters used in its production, material resistivity, strip width, or layer thickness. The values to be chosen will depend on the environmental conditions in which the detector will be placed, and the requirements in time resolution and gain, improving the detector performance for each given application. We present two different methods to calculate the propagation of charge diffusion through different resistive topologies; one is based on a FEM of solving the telegraph equation in our particular strip detector scheme, the other is based on a semi-analytical approach of charge diffusion and is used to determine the charge evolution in a resistive layer.",1304.2057v1 2014-07-31,Compact chromium oxide thin film resistors for use in nanoscale quantum circuits,"We report on the electrical characterisation of a series of thin chromium oxide films, grown by dc sputtering, to evaluate their suitability for use as on-chip resistors in nanoelectronics. By increasing the level of oxygen doping, the room-temperature sheet resistance of the chromium oxide films was varied from 28$\Omega / \square$ to 32.6k$\Omega / \square$. The variation in resistance with cooling to 4.2K in liquid helium was investigated; the sheet resistance at 4.2K varied with composition from 65$\Omega / \square$ to above 20G$\Omega / \square$. All of the films measured displayed ohmic behaviour at all measured temperatures. For on-chip devices for quantum phase-slip measurements using niobium-silicon nanowires, interfaces between niobium-silicon and chromium oxide are required. By characterising the interface contact resistance, we found that a gold intermediate layer is favourable: the specfic contact resistivity of chromium-oxide-to-gold interfaces was 0.15 m$\Omega$cm$^2$, much lower than the value for direct chromium-oxide to niobium-silicon interfaces, 65m$\Omega$cm$^2$. We conclude that these chromium oxide films are suitable for use in nanoscale circuits as high-value resistors, with resistivity tunable by oxygen content.",1407.8467v1 2016-06-12,Interlayer Resistance of Misoriented MoS2,"Interlayer misorientation in transition metal dichalcogenides alters the interlayer distance, the electronic band structure, and the vibrational modes, but, its effect on the interlayer resistance is not known. This work analyzes the coherent interlayer resistance of misoriented 2H-MoS2 for low energy electrons and holes as a function of the misorientation angle. The electronic interlayer resistance monotonically increases with the supercell lattice constant by several orders of magnitude similar to that of misoriented bilayer graphene. The large hole coupling gives low interlayer hole resistance that weakly depends on the misorientation angle. Interlayer rotation between an n-type region and a p-type region will suppress the electron current with little effect on the hole current. We estimate numerical bounds and explain the results in terms of the orbital composition of the bands at high symmetry points. Density functional theory calculations provide the interlayer coupling used in both a tunneling Hamiltonian and a non-equilibrium Green function calculation of the resistivity.",1606.03682v1 2017-11-30,Universal Scaling in Intrinsic Resistivity of Two-Dimensional Metal Borophene,"Two-dimensional boron sheets (borophenes) have been successfully synthesized in experiments and are expected to exhibit intriguing transport properties such as the emergence of superconductivity and Dirac Fermions. However, quantitative understanding of intrinsic electrical transport of borophene has not been achieved. Here, we report a comprehensive first-principles study on electron-phonon driven intrinsic electrical resistivity (\r{ho}) of emerging borophene structures. We find that the resistivity is highly dependent on the atomic structures and electron density of borophene. Low-temperature resistivity of borophene \r{ho} exhibits a universal scaling behavior, which increases rapidly with temperature T (\r{ho}~T^4), while \r{ho} increases linearly for a large temperature window T > 100 K. It is observed that this universal behavior of intrinsic resistivity is well described by Bloch-Gr\""unesisen model. Different from graphene and conventional three-dimensional metals, the intrinsic resistivity of borophenes can be easily tuned by adjusting carrier densities while the Bloch-Gr\""unesisen temperature is nearly fixed at ~100 K. Our work suggests monolayer boron can serve as an intriguing platform for realizing high-tunable two-dimensional electronic devices.",1711.11186v1 2018-05-05,Tetrahedral amorphous carbon resistive memories with graphene-based electrodes,"Resistive-switching memories are alternative to Si-based ones, which face scaling and high power consumption issues. Tetrahedral amorphous carbon (ta-C) shows reversible, non-volatile resistive switching. Here we report polarity independent ta-C resistive memory devices with graphene-based electrodes. Our devices show ON/OFF resistance ratios$\sim$4x$10^5$, ten times higher than with metal electrodes, with no increase in switching power, and low power density$\sim$14$\mu$W/$\mu$m$^2$. We attribute this to a suppressed tunneling current due to the low density of states of graphene near the Dirac point, consistent with the current-voltage characteristics derived from a quantum point contact model. Our devices also have multiple resistive states. This allows storing more than one bit per cell. This can be exploited in a range of signal processing/computing-type operations, such as implementing logic, providing synaptic and neuron-like mimics, and performing analogue signal processing in non-von-Neumann architectures",1805.02100v1 2017-03-10,Unipolar resistive switching in cobalt titanate thin films,"We report giant resistive switching of an order of 104, long-time charge retention characteristics up to 104 s, non-overlapping SET and RESET voltages, ohmic in low resistance state (LRS) and space charge limited current (SCLC) mechanism in high resistance state (HRS) properties in polycrystalline perovskite Cobalt Titanate (CoTiO3 ~ CTO) thin films. Impedance spectroscopy study was carried out for both LRS and HRS states which illustrates that only bulk resistance changes after resistance switching, however, there is a small change (<10% which is in pF range) in the bulk capacitance value in both states. These results suggest that in LRS state current filaments break the capacitor in many small capacitors in a parallel configuration which in turn provides the same capacitance in both states even there was 90 degree changes in phase-angle and an order of change in the tangent loss.",1703.03662v1 2015-04-21,The question of intrinsic origin of the metal-insulator transition in i-AlPdRe quasicrystal,"The icosahedral (i-) AlPdRe is the most resistive quasicrystalline alloy discovered so far. Resistivities ($\rho$) of $1\Omega cm$ at 4K and correlated resistance ratios ($RRR = \rho_{4K}/\rho_{300K}$) of more than 200 are observed in polycrystalline samples. These values are two orders of magnitude larger than for the isomorphous i-AlPdMn phase. We discuss here the controversial microscopic origin of the i-AlPdRe alloy electrical specificity. It has been proposed that the high resistivity values are due to extrinsic parameters, such as secondary phases or oxygen contamination. From comprehensive measurements and data from the literature including electronic transport correlated with micro structural and micro chemical analysis, we show that on the contrary there is mounting evidence in support of an origin intrinsic to the i-phase. Similarly to the other quasicrystalline alloys, the electrical resistivity of the i-AlPdRe samples depends critically on minute changes in the structural quality and chemical composition. The low resistivity in i-AlPdRe single-grains compared to polycrystaline samples can be explained by difference in chemical composition, heterogeneity and thermal treatment.",1504.05464v1 2023-04-08,Novel resistive charge-multipliers for dual-phase LAr-TPCs: towards stable operation at higher gains,"Cryogenic versions of Resistive WELL (RWELL) and Resistive Plate WELL (RPWELL) detectors have been developed, aimed at stable avalanche multiplication of ionization electrons in dual-phase TPCs. In the RWELL, a thin resistive layer deposited on top of an insulator is inserted in between the electron multiplier (THGEM) and the readout anode; in the RPWELL, a resistive plate is directly coupled to the THGEM. Radiation-induced ionization electrons in the liquid are extracted into the gaseous phase. They drift into the THGEM's holes where they undergo charge multiplication. Embedding resistive materials into the multiplier proved to enhance operation stability due to the mitigation of electrical discharges - thus allowing operation at higher charge gain compared to standard THGEM (a.k.a. LEM) multipliers. We present the detector concepts and report on the main preliminary results.",2304.04044v4 2012-02-10,What Causes High Resistivity in CdTe,"CdTe can be made semi-insulating by shallow donor doping. This is routinely done to obtain high resistivity in CdTe-based radiation detectors. However, it is widely believed that the high resistivity in CdTe is due to the Fermi level pinning by native deep donors. The model based on shallow donor compensation of native acceptors was dismissed based on the assumption that it is practically impossible to control the shallow donor doping level so precisely that the free carrier density can be brought below the desired value suitable for radiation detection applications. In this paper, we present our calculations on carrier statistics and energetics of shallow donors and native defects in CdTe. Our results show that the shallow donor can be used to reliably obtain high resistivity in CdTe. Since radiation detection applications require both high resistivity and good carrier transport, one should generally use shallow donors and shallow acceptors for carrier compensation and avoid deep centers that are effective carrier traps.",1202.2255v1 2003-05-17,Saturation of electrical resistivity,"Resistivity saturation is observed in many metallic systems with a large resistivity, i.e., when the resistivity has reached a critical value, its further increase with temperature is substantially reduced. This typically happens when the apparent mean free path is comparable to the interatomic separations - the Ioffe-Regel condition. Recently, several exceptions to this rule have been found. Here, we review experimental results and early theories of resistivity saturation. We then describe more recent theoretical work, addressing cases both where the Ioffe-Regel condition is satisfied and where it is violated. In particular we show how the (semiclassical) Ioffe-Regel condition can be derived quantum-mechanically under certain assumptions about the system and why these assumptions are violated for high-Tc cuprates and alkali-doped fullerides.",0305412v1 2004-07-06,"High pressure effects on the electrical resistivity behavior of the Kondo lattice, YbPd2Si2","We report the influence of external pressure (P= up to 8 GPa) on the temperature dependence of electrical resistivity of a Yb-based Kondo lattice, YbPd2Si2, which does not undergo magnetic ordering under ambient pressure condition. There are qualitative changes in the temperature dependence of electrical resistivity due to the application of external pressure. While the resistivity is found to vary quadratically below 15 K (down to 45 mK) characteristic of Fermi-liquids, a drop is observed below 0.5 K for P= 1 GPa. Since the resistance values do not attain zero, we are attempted to attribute this drop to magnetic ordering, rather than to superconductivity. The temperature at which this fall occurs goes through a peak as a function of P (8 K for2 GPa and about 5 K at higher pressures). mimicking Doniach's magnetic phase diagram. We conclude that this is one of the few Yb-based stoichiometric materials, in which one can travers from valence fluctuation to magnetic ordering by the application of external pressure.",0407125v1 2014-08-19,Effect of silicon resistivity on its porosification using metal induced chemical etching,"A comparison of porous structures formed from silicon (Si) wafers with different resistivities has been reported here based on the morphological studies carried out using scanning electron microscope (SEM). The porous Si samples have been prepared using metal induced etching (MIE) technique from two different Si wafers having two different resistivities. It is observed that porous Si containing well aligned Si nanowires are formed from high resistivity (1-20 $\Omega$cm) Si wafer whereas interconnected pores or cheese like structures are formed from low resistivity (0.02 $\Omega$cm ) Si wafers after MIE. An explanation for the different porosification processes has also been proposed based on the initial doping level where number of dopants seems to be playing an important role on the etching process. Visible photoluminescence have been observed from all the porous samples possibly due to quantum confinement effect.",1408.4314v1 2020-09-07,Tuneable Magneto-Resistance by Severe Plastic Deformation,"Bulk metallic samples were synthesized from different binary powder mixtures consisting of elemental Cu, Co, and Fe using severe plastic deformation. Small particles of the ferromagnetic phase originate in the conductive Cu phase, either by incomplete dissolution or by segregation phenomena during the deformation process. These small particles are known to give rise to granular giant magnetoresistance. Taking advantage of the simple production process, it is possible to perform a systematic study on the influence of processing parameters and material compositions on the magneto-resistance. Furthermore, it is feasible to tune the magnetoresistive behavior as a function of the specimens chemical composition. It was found that specimens of low ferromagnetic content show an almost isotropic drop in resistance in a magnetic field. With increasing ferromagnetic content, percolating ferromagnetic phases cause an anisotropy of the magnetoresistance. By changing the parameters of the high pressure torsion process, i.e., sample size, deformation temperature, and strain rate, it is possible to tailor the magnitude of giant magneto-resistance. A decrease in room temperature resistivity of approx. 3.5% was found for a bulk specimen containing an approximately equiatomic fraction of Co and Cu.",2009.02952v1 2017-11-22,High Efficiency Thin Film Superlattice Thermoelectric Cooler Modules Enabled by Low Resistivity Contacts,"V-telluride superlattice thin films have shown promising performance for on-chip cooling devices. Recent experimental studies have indicated that device performance is limited by the metal/semiconductor electrical contacts. One challenge in realizing a low resistivity contacts is the absence of fundamental knowledge of the physical and chemical properties of interfaces between metal and V-telluride materials. Here we present a combination of experimental and theoretical efforts to understand, design and harness low resistivity contacts to V-tellurides. Ab initio calculations are used to explore the effects of interfacial structure and chemical compositions on the electrical contacts, and an ab initio based macroscopic model is employed to predict the fundamental limit of contact resistivity as a function of both carrier concentration and temperature. Under the guidance of theoretical studies, we develop an experimental approach to fabricate low resistivity metal contacts to V-telluride thin film superlattices, achieving a 100-fold reduction compared to previous work. Interfacial characterization and analysis using both scanning transmission electron microscopy and energy-dispersive x-ray spectroscopy show the unusual interfacial morphology and the potential for further improvement in contact resistivity. Finally, we harness the improved contacts to realize an improved high-performance thermoelectric cooling module.",1711.08481v1 2000-02-17,Ion-Beam Induced Current in High-Resistance Materials,"The peculiarities of electric current in high-resistance materials, such as semiconductors or semimetals, irradiated by ion beams are considered. It is shown that after ion--beam irradiation an unusual electric current may arise directed against the applied voltage. Such a negative current is a transient effect appearing at the initial stage of the process. The possibility of using this effect for studying the characteristics of irradiated materials is discussed. A new method for defining the mean projected range of ions is suggested.",0002264v1 2021-11-15,Resistive-nanoindentation on gold: Experiments and modeling of the electrical contact resistance,"This paper reports the experimental, analytical, and numerical study of resistive-nanoindentation tests performed on gold samples (bulk and thin film). First, the relevant contributions to electrical contact resistance are discussed and analytically described. A brief comparison of tests performed on gold and on natively oxidized metals highlights the high reproducibility and the voltage-independence of experiments on gold(thanks to its oxide-free surface). Then, the evolution of contact resistance during nanoindentation is fully explained in terms of electronic transport regimes: starting from tunneling, electronic transport is then driven by ballistic conduction before ending with pure diffusive conduction. The corresponding analytical expressions, as well as their validity domains, are determined and compared with experimental data,showing excellent agreement. From there, focus is made on the diffusive regime. Resistive-nanoindentation outputs are fully described by analytical and finite-element modeling. The developed numerical framework allows a better understanding of the main parameters: it first assesses the technique capabilities (validity domains, sensitivity to tip defect, sensitivity to rheology, effect of an oxide layer, and so on), butit also validates the different assumptions made on current line distribution. Finally, it is shown that a simple calibration procedure allows a well-resolved monitoring of the contact area during resistive-nanoindentation performed on samples with complex rheologies (ductile thin film on an elastic substrate). Comparison to analytical and numerical approaches highlights the strength of resistive-nanoindentation for continuous area monitoring.",2111.15474v1 2023-08-09,Observation of abnormal resistance-temperature behavior along with diamagnetic transition in Pb$_{10-x}$Cu$_x$(PO$_4$)$_6$O-based composite,"Recently, Sukbae Lee et al.reported that material Pb$_{10-x}$Cu$_x$(PO$_4$)$_6$O (LK-99) has a series of characteristics of room temperature superconductors, including diamagnetic transition, resistance jump, nearly zero-resistance, magnetic field-dependent IV characteristics and so on (10.6111/JKCGCT.2023.33.2.061, arXiv:2307.12008, arXiv:2307.12037). However, whether LK-99 is really a room temperature superconductor is still controversial. On the one hand, some people think that the relatively weak diamagnetism of LK-99 reported by Sukbae Lee et al. is not the Meissner effect. On the other hand, there are doubts about the authenticity of its zero-resistance test results. Global replication studies have shown that LK-99 does have a large diamagnetic (arXiv:2308.01516), and also found a zero-resistance behavior at a low temperature of 110 $^\circ$K (arXiv:2308.01192). However, up to now, there is still no direct reproducible evidence to support Sukbae Lee et al.'s conclusion that LK-99 is a room temperature superconductor. Here, a distinct resistance jump was observed at about 387 $^\circ$K under ambient pressure in our experiment for unclear reason including possible impurity's contribution. The overall resistance of the test LK-99 sample still shows semiconductivity, and the resistance cannot really drop to zero. Our findings indicate that to identify the true potential of LK-99, high quality crystals without impurity are very important.",2308.05001v1 1995-12-14,Vortex structure and resistive transitions in high-Tc superconductors,"The nature of the resistive transition for a current applied parallel to the magnetic field in high-Tc materials is investigated by numerical simulation on the three dimensional Josephson junction array model. It is shown by using finite size scaling that for samples with disorder the critical temperature Tp for the c axis resistivity corresponds to a percolation phase transition of vortex lines perpendicularly to the applied field. The value of Tp is higher than the critical temperature for j perpendicular to H, but decreases with the thickness of the sample and with anisotropy. We predict that critical behavior around Tp should reflect in experimentally accessible quantities, as the I-V curves.",9512003v1 2010-06-26,Stabilizing the forming process in unipolar resistance switching using an improved compliance current limiter,"The high reset current IR in unipolar resistance switching now poses major obstacles to practical applications in memory devices. In particular, the first IR-value after the forming process is so high that the capacitors sometimes do not exhibit reliable unipolar resistance switching. We found that the compliance current Icomp is a critical parameter for reducing IR-values. We therefore introduced an improved, simple, easy to use Icomp-limiter that stabilizes the forming process by drastically decreasing current overflow, in order to precisely control the Icomp- and subsequent IR-values.",1006.5132v1 2011-07-06,Hysteretic magnetic pinning and reversible resistance switching in High-Tc superconductor/ferromagnet multilayers,"We study a high-TC superconducting (YBa2Cu3O7-d) / ferromagnetic (Co/Pt multilayer) hybrid which exhibits resistance switching driven by the magnetic history: depending on the direction of the external field, a pronounced decrease or increase of the mixed-state resistance is observed as magnetization reversal occurs within the Co/Pt multilayer. We demonstrate that stray magnetic fields cause these effects via i) creation of vortices/antivortices and ii) magnetostatic pinning of vortices that are induced by the external field.",1107.1122v1 2017-05-11,The role of contact resistance in graphene field-effect devices,"The extremely high carrier mobility and the unique band structure, make graphene very useful for field-effect transistor applications. According to several works, the primary limitation to graphene based transistor performance is not related to the material quality, but to extrinsic factors that affect the electronic transport properties. One of the most important parasitic element is the contact resistance appearing between graphene and the metal electrodes functioning as the source and the drain. Ohmic contacts to graphene, with low contact resistances, are necessary for injection and extraction of majority charge carriers to prevent transistor parameter fluctuations caused by variations of the contact resistance. The International Technology Roadmap for Semiconductors, toward integration and down-scaling of graphene electronic devices, identifies as a challenge the development of a CMOS compatible process that enables reproducible formation of low contact resistance. However, the contact resistance is still not well understood despite it is a crucial barrier towards further improvements. In this paper, we review the experimental and theoretical activity that in the last decade has been focusing on the reduction of the contact resistance in graphene transistors. We will summarize the specific properties of graphene-metal contacts with particular attention to the nature of metals, impact of fabrication process, Fermi level pinning, interface modifications induced through surface processes, charge transport mechanism, and edge contact formation.",1705.04025v1 2022-09-13,Unconventional Resistivity Scaling in Topological Semimetal CoSi,"Nontrivial band topologies in semimetals lead to robust surface states that can contribute dominantly to the total conduction. This may result in reduced resistivity with decreasing feature size contrary to conventional metals, which may highly impact the semiconductor industry. Here we study the resistivity scaling of a representative topological semimetal CoSi using realistic band structures and Green's function methods. We show that there exists a critical thickness d_c dividing different scaling trends. Above d_c, when the defect density is low such that surface conduction dominates, resistivity reduces with decreasing thickness; when the defect density is high such that bulk conduction dominates, resistivity increases in as conventional metals. Below d_c, the persistent remnants of the surface states give rise to decreasing resistivity down to the ultrathin limit, unlike in topological insulators. The observed CoSi scaling can apply to broad classes of topological semimetals, providing guidelines for materials screening and engineering. Our study shows that topological semimetals bear the potential of overcoming the resistivity scaling challenges in back-end-of-line interconnect applications.",2209.06135v1 2019-10-31,Tackling Challenges in Seebeck Coefficient Measurement of Ultra-High Resistance Samples with an AC Technique,"Seebeck coefficient is a widely-studied semiconductor property. Conventional Seebeck coefficient measurements are based on DC voltage measurement. Normally this is performed on samples with low resistances below a few Mohm level. Meanwhile, certain semiconductors are highly intrinsic and resistive, many examples can be found in optical and photovoltaic materials. The hybrid halide perovskites that have gained extensive attention recently are a good example. Few credible studies exist on the Seebeck coefficient of, CH3NH3PbI3, for example. We report here an AC technique based Seebeck coefficient measurement, which makes high quality voltage measurement on samples with resistances up to 100Gohm. This is achieved through a specifically designed setup to enhance sample isolation and reduce meter loading. As a demonstration, we performed Seebeck coefficient measurement of a CH3NH3PbI3 thin film at dark and found S = +550 microV/K. Such property of this material has not been successfully studied before.",1910.14205v1 2021-04-03,Resistive switching of tetraindolyl derivative in ultrathin films: A potential candidate for non-volatile memory applications,"Bipolar resistive switching using organic molecule is very promising for memory application owing to their advantages like simple device structure, low manufacturing cost, their stability and flexibility etc. Herein we report Langmuir-Blodgett and spin-coated film based bipolar resistive switching devices using organic material indole derivative. Pressure - area per molecule isotherm, Brewster Angle Microscopy, Atomic Force Microscopy and Scanning Electron Microscopy were used to have an idea about organization and morphology of the organic material onto thin film. Based on device structure and measurement protocol it is observed that the device made up of 1 shows non-volatile Resistive Random Access Memory behaviour with very high memory window, data sustainability and repeatability.Oxidation-reduction process as well as electric field driven conduction are the key behind such switching behaviour.Due to very good data retention, repeatability, stability and high device yield the switching device designed using compound 1may be a potential candidate for memory applications.",2104.01298v1 2021-06-05,On the anomalous low-resistance state and exceptional Hall component in hard-magnetic Weyl nanoflakes,"Magnetic topological materials, which combine magnetism and topology, are expected to host emerging topological states and exotic quantum phenomena. In this study, with the aid of greatly enhanced coercive fields in high-quality nanoflakes of the magnetic Weyl semimetal Co3Sn2S2, we investigate anomalous electronic transport properties that are difficult to reveal in bulk Co3Sn2S2 or other magnetic materials. When the magnetization is antiparallel to the applied magnetic field, the low longitudinal resistance state occurs, which is in sharp contrast to the high resistance state for the parallel case. Meanwhile, an exceptional Hall component that can be up to three times larger than conventional anomalous Hall resistivity is also observed for transverse transport. These anomalous transport behaviors can be further understood by considering nonlinear magnetic textures and the chiral magnetic field associated with Weyl fermions, extending the longitudinal and transverse transport physics and providing novel degrees of freedom in the spintronic applications of emerging topological magnets.",2106.02906v1 2023-08-30,Chemical heterogeneity enhances hydrogen resistance in high-strength steels,"When H, the lightest, smallest and most abundant atom in the universe, makes its way into a high-strength alloy (>650 MPa), the material's load-bearing capacity is abruptly lost. This phenomenon, known as H embrittlement, was responsible for the catastrophic and unpredictable failure of large engineering structures in service. The inherent antagonism between high strength requirements and H embrittlement susceptibility strongly hinders the design of lightweight yet reliable structural components needed for carbon-free hydrogen-propelled industries and reduced-emission transportation solutions. Inexpensive and scalable alloying and microstructural solutions that enable both, an intrinsically high resilience to H and high mechanical performance, must be found. Here we introduce a counterintuitive strategy to exploit typically undesired chemical heterogeneity within the material's microstructure that allows the local enhancement of crack resistance and local H trapping, thereby enhancing the resistance against H embrittlement. We deploy this approach to a lightweight, high-strength steel and produce a high-number density Mn-rich zones dispersed within the microstructure. These solute-rich buffer regions allow for local micro-tuning of the phase stability, arresting H-induced microcracks thus interrupting the H-assisted damage evolution chain, regardless of how and when H is introduced and also regardless of the underlying embrittling mechanisms. A superior H embrittlement resistance, increased by a factor of two compared to a reference material with a homogeneous solute distribution within each microstructure constituent, is achieved at no expense of the material's strength and ductility.",2308.16048v1 2021-01-29,Novel design strategies for modulating conductive stretchable system response based on periodic assemblies,"Soft electronics have recently gathered considerable interest thanks to their bio-mechanical compatibility. An important feature of such deformable conductors is their electrical response to strain. While development of stretchable materials with high gauge factors has attracted considerable attention, there is a growing need for stretchable conductors whose response to deformation can be accurately engineered to provide arbitrary resistance-strain relationships. The rare studies addressing this issue have focused on deterministic geometries of single rigid materials, limiting the scope of such strategies. Herein, we introduce the novel concept of periodic stretchable patterns combining multiple conductive materials to produce tailored responses. Using shortest-path algorithms, we establish a computationally efficient selection method to obtain required resistance-strain relationship. Using this algorithm, we identify and experimentally demonstrate constant resistance-strain responses up to 50% elongation using a single micro-textured material. Finally, we demonstrate counter-intuitive sinusoidal responses by integrating three materials, with interesting applications in sensing and soft robotics.",2101.12600v1 2009-03-07,Correlation between resistance fluctuations and temperature dependence of conductivity in graphene,"The weak temperature dependence of the resistance R(T) of monolayer graphene1-3 indicates an extraordinarily high intrinsic mobility of the charge carriers. Important complications are the presence of mobile scattering centres that strongly modify charge transport, and the presence of strong mesoscopic conductance fluctuations that, in graphene, persist to relatively high temperatures4,5. In this Letter, we investigate the surprisingly varied changes in resistance that we find in graphene flakes as temperature is lowered below 70 K. We propose that these changes in R(T) arise from the temperature dependence of the scattered electron wave interference that causes the resistance fluctuations. Using the field effect transistor configuration, we verify this explanation in detail from measurements of R(T) by tuning to different gate voltages corresponding to particular features of the resistance fluctuations. We propose simple expressions that model R(T) at both low and high charge carrier densities.",0903.1334v1 2021-04-20,Accelerated Discovery of Molten Salt Corrosion-resistant Alloy by High-throughput Experimental and Modeling Methods Coupled to Data Analytics,"Insufficient availability of molten salt corrosion-resistant alloys severely limits the fruition of a variety of promising molten salt technologies that could otherwise have significant societal impacts. To accelerate alloy development for molten salt applications and develop fundamental understanding of corrosion in these environments, here we present an integrated approach using a set of high-throughput alloy synthesis, corrosion testing, and modeling coupled with automated characterization and machine learning. By using this approach, a broad range of Cr-Fe-Mn-Ni alloys were evaluated for their corrosion resistances in molten salt simultaneously demonstrating that corrosion-resistant alloy development can be accelerated by thousands of times. Based on the obtained results, we unveiled a sacrificial mechanism in the corrosion of Cr-Fe-Mn-Ni alloys in molten salts which can be applied to protect the less unstable elements in the alloy from being depleted, and provided new insights on the design of high-temperature molten salt corrosion-resistant alloys.",2104.10235v1 2014-12-05,Resistance switching devices based on amorphous insulator-metal thin films,"Nanometallic devices based on amorphous insulator-metal thin films are developed to provide a novel non-volatile resistance-switching random-access memory (RRAM). In these devices, data recording is controlled by a bipolar voltage, which tunes electron localization length, thus resistivity, through electron trapping/detrapping. The low-resistance state is a metallic state while the high-resistance state is an insulating state, as established by conductivity studies from 2K to 300K. The material is exemplified by a Si3N4 thin film with randomly dispersed Pt or Cr. It has been extended to other materials, spanning a large library of oxide and nitride insulator films, dispersed with transition and main-group metal atoms. Nanometallic RRAMs have superior properties that set them apart from other RRAMs. The critical switching voltage is independent of the film thickness/device area/temperature/switching speed. Trapped electrons are relaxed by electron-phonon interaction, adding stability which enables long-term memory retention. As electron-phonon interaction is mechanically altered, trapped electron can be destabilized, and sub-picosecond switching has been demonstrated using an electromagnetically generated stress pulse. AC impedance spectroscopy confirms the resistance state is spatially uniform, providing a capacitance that linearly scales with area and inversely scales with thickness. The spatial uniformity is also manifested in outstanding uniformity of switching properties. Device degradation, due to moisture, electrode oxidation and dielectrophoresis, is minimal when dense thin films are used or when a hermetic seal is provided. The potential for low power operation, multi-bit storage and complementary stacking have been demonstrated in various RRAM configurations.",1412.2083v1 2003-11-05,"Thermoelectric power of Bi and Bi(1-x)Te(x), x=0.0014,in porous Vycor glass","Semiconductor quantum wires constitute a promising thermoelectric material because of the increase of the electronic density of states in low-dimensional materials. We studied the magnetic-field-dependent resistance and Seebeck coefficient of a high-density network of 6-nm-diameter wires of Bi and of Bi(1-x)Te(x), x=0.0014, in porous Vycor glass. The resistance R increases as temperature decreases from 300 K down to 0.3 K for both composites. However, in contrast to recent results that demonstrate the semiconducting behavior of the resistance and very large enhancements of the thermoelectric power of composites containing Bi nanowires with diameters of 9 and 15 nm, we find that the resistance is not thermally activated and that the thermoelectric power of the composites is of the same order of magnitude as the thermoelectric power of bulk Bi. Our results are consistent with the nanowires having carrier density that is enhanced by surface effects.",0311112v1 2009-06-27,Resistive switching in nanogap systems on SiO2 substrates,"Voltage-controlled resistive switching is demonstrated in various gap systems on SiO2 substrate. The nanosized gaps are made by different means using different materials including metal, semiconductor, and metallic nonmetal. The switching site is further reduced by using multi-walled carbon nanotubes and single-walled carbon nanotubes. The switching in all the gap systems shares the same characteristics. This independence of switching on the material compositions of the electrodes, accompanied by observable damage to the SiO2 substrate at the gap region, bespeaks the intrinsic switching from post-breakdown SiO2. It calls for caution when studying resistive switching in nanosystems on oxide substrates, since oxide breakdown extrinsic to the nanosystem can mimic resistive switching. Meanwhile, the high ON/OFF ratio (10E5), fast switching time (2 us, test limit), durable cycles demonstrated show promising memory properties. The intermediate states observed reveal the filamentary conduction nature.",0906.5100v1 2010-02-12,Experimental Study of Resistive Bistability in Metal Oxide Junctions,"We have studied resistive bistability (memory) effects in junctions based on metal oxides, with a focus on sample-to-sample reproducibility which is necessary for the use of such junctions as crosspoint devices of hybrid CMOS/nanoelectronic circuits. Few-nm-thick layers of NbOx, CuOx and TiOx have been formed by thermal and plasma oxidation, at various deposition and oxidation conditions, both with or without rapid thermal post-annealing (RTA). The resistive bistability effect has been observed for all these materials, with particularly high endurance (over 1000 switching cycles) obtained for single-layer TiO2 junctions, and the best reproducibility reached for multi-layer junctions of the same material. Fabrication optimization has allowed us to improve the OFF/ON resistance ratio to about 1000, but the sample-to-sample reproducibility is so far lower than that required for large scale integration.",1002.2650v1 2018-03-30,Reliability assessment in advanced nanocomposite materials for orthopaedic applications,"Alumina-zirconia nano-composites were recently developed as alternative bearing materials for orthopedics. Previous, preliminary reports show that such alumina-zirconia nanocomposites exhibit high crack resistance and low wear rate. In this paper, additional information is given in terms of wear, crack resistance and ageing behaviour: femoral heads are inspected after 7 million cycles of wear testing on a hip simulator, crack resistance is measured and compared to other ceramics used today in orthopedics, slow crack growth is reported under static and cyclic fatigue, and aging resistance is assessed. We also report on the load to failure of femoral heads prototypes during compression tests. This overall reliability assessment ensures a potential future development for these kinds of new nanocomposites in the orthopedic field.",1804.08702v1 2018-10-18,Topological Hall effect in thin films of Mn$_{1.5}$PtSn,"Spin chirality in metallic materials with non-coplanar magnetic order can give rise to a Berry phase induced topological Hall effect. Here, we report the observation of a large topological Hall effect in high-quality films of Mn$_{1.5}$PtSn that were grown by means of magnetron sputtering on MgO(001). The topological Hall resistivity is present up to $\mu_{0}H \approx 4~$T below the spin reorientation transition temperature, $T_{s}=185$~K. We find, that the maximum topological Hall resistivity is of comparable magnitude as the anomalous Hall resistivity. Owing to the size, the topological Hall effect is directly evident prior to the customarily performed subtraction of magnetometry data. Further, we underline the robustness of the topological Hall effect in Mn\textsubscript{2-x}PtSn by extracting the effect for multiple stoichiometries (x~=~0.5, 0.25, 0.1) and film thicknesses (t = 104, 52, 35~nm) with maximum topological Hall resistivities between $0.76~\mu\Omega$cm and $1.55~\mu\Omega$cm at 150~K.",1810.08232v1 2019-06-19,Origin of current-controlled negative differential resistance modes and the emergence of composite characteristics with high complexity,"Current-controlled negative differential resistance has significant potential as a fundamental building block in brain-inspired neuromorphic computing. However, achieving desired negative differential resistance characteristics, which is crucial for practical implementation, remains challenging due to little consensus on the underlying mechanism and unclear design criteria. Here, we report a material-independent model of current-controlled negative differential resistance to explain a broad range of characteristics, including the origin of the discontinuous snap-back response observed in many transition metal oxides. This is achieved by explicitly accounting for a non-uniform current distribution in the oxide film and its impact on the effective circuit of the device, rather than a material-specific phase transition. The predictions of the model are then compared with experimental observations to show that the continuous S-type and discontinuous snap-back characteristics serve as fundamental building blocks for composite behaviour with higher complexity. Finally, we demonstrate the potential of our approach for predicting and engineering unconventional compound behaviour with novel functionality for emerging electronic and neuromorphic computing applications.",1907.02651v1 2022-05-06,Interfacial resistive switching by multiphase polarization in ion-intercalation nanofilms,"Nonvolatile resistive-switching (RS) memories promise to revolutionize hardware architectures with in-memory computing. Recently, ion-interclation materials have attracted increasing attention as potential RS materials for their ion-modulated electronic conductivity. In this Letter, we propose RS by multiphase polarization (MP) of ion-intercalated thin films between ion-blocking electrodes, in which interfacial phase separation triggered by an applied voltage switches the electron-transfer resistance. We develop an electrochemical phase-field model for simulations of coupled ion-electron transport and ion-modulated electron-transfer rates and use it to analyze the MP switching current and time, resistance ratio, and current-voltage response. The model is able to reproduce the complex cyclic voltammograms of lithium titanate (LTO) memristors, which cannot be explained by existing models based on bulk dielectric breakdown. The theory predicts the achievable switching speeds for multiphase ion-intercalation materials and could be used to guide the design of high-performance MP-based RS memories.",2205.02980v2 2023-09-13,Amorphous VO$_x$ films with high temperature coefficient of the resistivity grown by reactive e-beam evaporation of V metal,"Amorphous VO$_x$ films without a hysteretic phase transition are stable with respect to thermal cycling and highly demanded as sensitive elements of the resistive thermometers and microbolometers. In this paper we present simple and low-temperature growth of amorphous vanadium oxide films by reactive electron beam evaporation of vanadium metal in $\sim 10^{-4}$ mBar oxygen atmosphere. The temperature coefficient of the resistivity (TCR) of the films is weakly sensitive to substrate material and temperature and could be tuned by oxygen pressure in the growth chamber up to -2.2\% /K. The resistivity value is stable for months. It depends on the substrate material and substrate temperature during the evaporation. Simplicity and controllability of the method should lead to various laboratory and industrial applications.",2309.07036v1 2007-01-02,Negative Differential Resistance of Electrons in Graphene Barrier,"The graphene is a native two-dimensional crystal material consisting of a single sheet of carbon atoms. In this unique one-atom-thick material, the electron transport is ballistic and is described by a quantum relativistic-like Dirac equation rather than by the Schrodinger equation. As a result, a graphene barrier behaves very differently compared to a common semiconductor barrier. We show that a single graphene barrier acts as a switch with a very high on-off ratio and displays a significant differential negative resistance, which promotes graphene as a key material in nanoelectronics.",0701011v1 2019-10-07,Growth and Characterization of Polycrystalline NbO2 Thin Films on Crystalline and Amorphous Substrates,"NbO2 is a potential material for nanometric memristor devices, both in the amorphous and the crystalline form. We fabricated NbO2 thin films using RF-magnetron sputtering from a stoichiometric target. The as-deposited films were amorphous regardless of the sputtering parameters. Post deposition vacuum annealing of the films was necessary to achieve crystallinity. A high degree of crystallinity was obtained by optimizing annealing duration and temperature. The resistivity of the material increases as it undergoes a structural transition from amorphous to crystalline with the crystalline films being one order of magnitude more resistive.",1910.02824v1 2004-04-18,Anisotropy of superconductivity of as-grown MgB$_2$ thin films by molecular beam epitaxy,"Superconducting thin films of magnesium diboride (MgB$_2$) were prepared on MgO (001) substrate by a molecular beam epitaxy (MBE) method with the co-evaporation conditions of low deposition rate in ultra-high vacuum. The structural and physical properties of the films were studied by RHEED, XRD, XPS, resistivity and magnetization measurements.All films demonstrated superconductivity without use of any post-annealing process.The highest {\it T}$_{c,onset}$ determined by resistivity measurement was about 33K in the present samples.Anisotropic superconducting properties were evaluated by the resistivity and magnetic measurements.We will discuss the anisotropy of superconductivity for as-grown MgB$_2$ thin films.",0404415v1 2005-08-02,Epitaxial growth and transport properties of Nb-doped SrTiO$_{3}$ thin films,"Nb-doped SrTiO$_{3}$ epitaxial thin films have been prepared on (001) SrTiO$_{3}$ substrates using pulsed laser deposition. A high substrate temperature ($>1000^{\circ}{C}$) was found to be necessary to achieve 2-dimensional growth. Atomic force microscopy reveals atomically flat surfaces with 3.9 \AA $ $ steps. The films show a metallic behavior, residual resistivity ratios between 10 and 100, and low residual resistivity of the order of 10$^{-4}$$\Omega$cm. At 0.3 K, a sharp superconducting transition, reaching zero resistance, is observed.",0508073v1 2011-11-07,Monte Carlo Study of Magnetic Resistivity in Semiconducting MnTe,"We investigate in this paper properties of the spin resistivity in the magnetic semiconducting MnTe of NiAs structure. MnTe is a crossroad semiconductor with a large band gap. It is an antiferromagnet with the N\'eel temperature around 310K. Due to this high N\'eel temperature, there are many applications using its magnetic properties. The method we use here is the Monte Carlo simulation in which we take into account the interaction between itinerant spins and lattice Mn spins. Our results show a very good agreement with experiments on the shape of the spin resistivity near the N\'eel temperature.",1111.1507v1 2016-11-21,Ramsey Interferometry of Particle-Hole Pairs in Tunnel Junctions,"We present a method to probe real-time dynamics in quantum mesoscopic systems using Ramsey interferometry. This allows us to explore the effect of interactions on quasi-particles in the time domain. We investigate the dephasing effects of an ohmic environment on an electron-hole pair in a tunnel junction. We show that dynamical Coulomb blockade phenomena can be observed for resistances much smaller than the quantum of resistance. Moreover, the crossover between high and low impedance limits can be probed for a constant resistance by a proper control of the voltage modulation.",1611.06738v1 2010-11-08,Normal state resistivity of Ba$_{1-x}$K$_x$Fe$_2$As$_2$: evidence for multiband strong-coupling behavior,"We present theoretical analysis of the normal state resistivity in multiband superconductors in the framework of Eliashberg theory. The results are compared with measurements of the temperature dependence of normal state resistivity of high-purity Ba$_{0.68}$K$_{0.32}$Fe$_{2}$As$_{2}$ single crystals with the highest reported transition temperature $T_c$ = 38.5 K. The experimental data demonstrate strong deviations from the Bloch-Gr\""{u}neisen behavior, namely the tendency to saturation of the resistivity at high temperatures. The observed behavior of the resistivity is explained within the two band scenario when the first band is strongly coupled and relatively clean, while the second band is weakly coupled and is characterized by much stronger impurity scattering.",1011.1900v3 2014-03-18,Electron-Phonon Interactions and the Intrinsic Electrical Resistivity of Graphene,"We present a first-principles study of the temperature- and density-dependent intrinsic electrical resistivity of graphene. We use density-functional theory and density-functional perturbation theory together with very accurate Wannier interpolations to compute all electronic and vibrational properties and electron-phonon coupling matrix elements; the phonon-limited resistivity is then calculated within a Boltzmann-transport approach. An effective tight-binding model, validated against first-principles results, is also used to study the role of electron-electron interactions at the level of many-body perturbation theory. The results found are in excellent agreement with recent experimental data on graphene samples at high carrier densities and elucidate the role of the different phonon modes in limiting electron mobility. Moreover, we find that the resistivity arising from scattering with transverse acoustic phonons is 2.5 times higher than that from longitudinal acoustic phonons. Last, high-energy, optical, and zone-boundary phonons contribute as much as acoustic phonons to the intrinsic electrical resistivity even at room temperature and become dominant at higher temperatures.",1403.4603v1 2018-06-03,Influence of hydrogen on electron-phonon coupling and intrinsic electrical resistivity in zirconium: a first-principles study,"The paper presents the first-principle calculation of the electron-phonon coupling and the temperature dependence of the intrinsic electrical resistivity of the zirconium-hydrogen system with various hydrogen concentrations. The nature of the anomalous decrease in the electrical resistivity of the Zr-H system with the increase of hydrogen concentration (at the high concentrations of H/Zr$>$1.5) was studied. It was found that the hydrogen concentration, where the resistivity starts to decrease, is very close to the critical concentration of the $\delta-\varepsilon$ phase transition. It was shown that the tetragonal lattice distortion due to the $\delta-\varepsilon$ phase transition of the Zr-H system eliminates imaginary phonon frequencies and the strong electron-phonon coupling of the $\delta$ phase and, as a result, leads to the reduction of the electrical resistivity of the Zr-H system at a high hydrogen concentration.",1806.00847v3 2021-12-29,Significant reduction in semiconductor interface resistance via interfacial atomic mixing,"The contact resistance between two dissimilar semiconductors is determined by the carrier transmission through their interface. Despite the ubiquitous presence of interfaces, quantitative simulation of charge transport across such interfaces is difficult, limiting the understanding of interfacial charge transport. This work employs Green's functions to study the charge transport across representative Si/Ge interfaces. For perfect interfaces, it is found that the transmittance is small and the contact resistance is high, not only because the mismatch of carrier pockets makes it hard to meet the momentum conservation requirement, but also because of the incompatible symmetries of the Bloch wave functions of the two sides. In contrast, atomic mixing at the interface increases the carrier transmittance as the interface roughness opens many nonspecular transmission channels, which greatly reduces the contact resistance compared with the perfect interface. Specifically, we show that disordered interfaces with certain symmetries create more nonspecular transmission. The insights from our study will benefit the future design of high-performance heterostructures with low contact resistance.",2112.14400v2 2005-02-26,Josephson junction decoupling is the main origin of AC resistivity in the superconducting state,"The origin of AC resistivity in the high Tc superconductors is not addressed adequately in literature. We found out, Josephson Junction (JJ) decoupling is the main origin of the AC resistivity in high Tc superconductors. We have measured the AC resistivity in the superconductors in the low frequency range by measuring the complex AC impedance of superconducting YBa2Cu3O7 (YBCO) polycrystalline samples. Our data shows that under certain conditions when the number density of Josephson Junctions (JJ) present in the sample and the JJ critical current crosses a threshold value, AC resistivity in the superconducting state keeps on increasing with lowering temperature. The underlying mechanism is an interesting interplay of JJ coupling energy, amplitude of the supply AC voltage and the current applied to the superconducting sample. The effect of the applied AC current of different frequencies and the variation of temperature were studied in detail. To find out the exact relation between the JJ coupling energy, JJ number density, applied AC frequency, the amplitude of AC current and the AC resistivity in the superconductors, we have studied samples of different grain sizes, pressurized with different pressure and sintered at different physical situations. These results have important implications for the understanding of the origin of AC resistivity and characterization of superconducting samples. In this paper we also extend the capability of the AC impedance studies in superconductors for the characterization of materials for device applications.",0502639v1 2022-08-03,Low Resistance Ohmic Contact On Epitaxial MOVPE-grown $β$-Ga$_2$O$_3$ and $β$-(Al$_x$Ga$_1-x$)$_2$ O$_3$ Films,"We report on the realization of record low resistance Ohmic contacts to MOVPE-grown heavily Si-doped $\beta$-Ga$_2$O$_3$ and $\beta$-(Al$_x$Ga$_1-x$)$_2$ O$_3$ epitaxial films. Transfer length measurement (TLM) patterns were fabricated on the heavily Si-doped homoepitaxial $\beta$-Ga$_2$O$_3$ films with electron concentration (n) ranging from 1.77 to 3.23e20 cm^-3. Record low specific contact resistance and total contact resistance (Rc) of 1.62e-7 Ohm.cm^2 and 0.023 Ohm.mm were realized for $\beta$-Ga$_2$O$_3$: Si films with n > 3e20 cm^-3. TLM structures were also fabricated on heavily Si doped coherently strained $\beta$-(Al$_x$Ga$_1-x$)$_2$ O$_3$ (x=12%, 17% and 22%) films. The film with 12% Al composition (n=1.23e20 cm^-3) showed \r{ho}c of 5.85e-6 Ohm.cm^2, but it increased to 2.19e-4 Ohm.cm^2 for a layer with a 22% Al composition. Annealing the samples post metal deposition has generally led to a decrease in contact resistance, but for high Al content $\beta$-(Al$_x$Ga$_1-x$)$_2$ O$_3$, the contact resistance did not change significantly after the annealing process. The low contact resistance values measured in this work are very promising for the fabrication of high frequency power devices.",2208.02322v1 2022-11-30,High-efficiency energy harvesting based on nonlinear Hall rectifier,"Noncentrosymmetric quantum materials can convert AC input current into DC transverse current through the nonlinear Hall effect at zero magnetic field. We analyze the AC-DC power conversion efficiency of such ``Hall rectifier'' and suggest its application in wireless charging and energy harvesting. Our key observation is that the development of Hall voltage results in a change of longitudinal resistance, resulting in a violation of Ohm's law due to the nonlinear Hall effect. This feedback mechanism balances the input power and the output power and hence is crucial to understanding the power transfer from source to load. We derive a general expression for the power conversion efficiency in terms of material parameters, external load resistance, and input power. As the Hall current is perpendicular to the electric field and does not generate Joule heating by itself, we obtain high power conversion efficiency when the Hall angle (which increases with the input power) is large and the load resistance is optimized. Promising materials for high-efficiency Hall rectifiers are also discussed.",2211.17219v2 2011-02-28,Introduction to bulk metallic glass composite and its recent applications,"Bulk metallic glass (BMG) materials are hot topics in recent years, not to mention BMG matrix composites, which further improve the magnetic and mechanical properties of BMG materials. BMG and BMG matrix materials are fast developing and promising materials in modern industry due to their extraordinary properties such as high strength, low density, excellent resistibility to high temperature and corrosion. In this paper, I reviewed processing and application of several recently developed BMG and BMG matrix materials.",1102.5758v1 2008-05-04,Increase of the wear resistance of carbide layers deposited by Pulsed Laser Deposition in addition with an auxiliary laser,"Carbides stand out because of their high hardness and wear-resistance. Thus these materials are often discussed for coatings of machine tools etc. Within this work Boron Carbide (B4C) and Carbide (C) thin films were deposited on Si (100) substrates by pulsed-laser deposition technique. In order to improve the wear-resistance of the deposited films, we introduced a new working technique including the application of a second excimer laser in a special working mode. Thereby one laser was used to ablate the carbide material from a target and to deposit the material on the substrate. The light of the second laser was directed directly onto the substrate in order to modify the ablated material. We report on details for film deposition and film properties determined by Scanning Electron Microscope, Energy Dispersive X-Ray Spectroscopy, X-Ray Diffraction, Rutherford Backscattering, Raman Spectroscopy and tribological experiments.",0805.0430v1 2017-10-24,Lithographic performance of ZEP520A and mr-PosEBR resists exposed by electron beam and extreme ultraviolet lithography,"Pattern transfer by deep anisotropic etch is a well-established technique for fabrication of nanoscale devices and structures. For this technique to be effective, the resist material plays a key role and must have high resolution, reasonable sensitivity and high etch selectivity against the conventional silicon substrate or underlayer film. In this work, the lithographic performance of two high etch resistance materials was evaluated: ZEP520A (Nippon Zeon Co.) and mr-PosEBR (micro resist technology GmbH). Both materials are positive tone, polymer-based and non-chemically amplified resists. Two exposure techniques were used: electron beam lithography (EBL) and extreme ultraviolet (EUV) lithography. These resists were originally designed for EBL patterning, where high quality patterning at sub-100 nm resolution was previously demonstrated. In the scope of this work, we also aim to validate their extendibility to EUV for high resolution and large area patterning. To this purpose, the same EBL process conditions were employed at EUV. The figures of merit, i.e. dose to clear, dose to size, and resolution, were extracted and these results are discussed systematically. It was found that both materials are very fast at EUV (dose to clear lower than 12 mJ/cm2) and are capable of resolving dense lines/space arrays with a resolution of 25 nm half-pitch. The quality of patterns was also very good and the sidewall roughness was below 6 nm. Interestingly, the general-purpose process used for EBL can be extended straightforwardly to EUV lithography with comparable high quality and yield. Our findings open new possibilities for lithographers who wish to devise novel fabrication schemes exploiting EUV for fabrication of nanostructures by deep etch pattern transfer.",1710.08733v1 2016-04-14,Study of Glass and Bakelite properties as electrodes in RPCs,"India-based Neutrino Observatory (INO) collaboration is planning to build a magnetized Iron-CALorimeter detector (ICAL) for the study of atmospheric neutrinos. ICAL detector will be a stack of 151 layers of magnetized iron plates interleaved with Resistive Plate Chambers (RPCs) as active detector elements with a total mass of 50 kton. Resistive Plate Chambers are gaseous detectors made up of two parallel electrodes of high bulk resistivity like float glass and bakelite. These detectors are extensively used in several high energy physics experiments since 1980s because of high count rate, excellent time as well as spatial resolutions, simple to fabricate and operate. Due to detector aging issue, it is necessary to characterize electrode material so as to select appropriate electrode material before fabricating the detector. In the present studies, we measured bulk resistivity and surface current of glass as well as bakelite. Bulk resistivity of bakelite is ~ 100 times less than that of glass and surface current of bakelite is higher than that of glass. Also glass does not need any kind of surface treatment to achieve better surface uniformity. Therefore, glass electrodes are preferred over bakelite electrodes in most of the cases. Locally manufactured Asahi glass of ~2 mm thickness and bakelite sheets were tested during the studies as reported in this paper before the various stages of detector fabrication.",1604.04130v2 2023-01-11,Resistive Switching and Current Conduction Mechanisms in Hexagonal Boron Nitride Threshold Memristors with Nickel Electrodes,"The two-dimensional (2D) insulating material hexagonal boron nitride (h BN) has attracted much attention as the active medium in memristive devices due to its favorable physical properties, among others, a wide bandgap that enables a large switching window. Metal filament formation is frequently suggested for h-BN devices as the resistive switching (RS) mechanism, usually supported by highly specialized methods like conductive atomic force microscopy (C-AFM) or transmission electron microscopy (TEM). Here, we investigate the switching of multilayer hexagonal boron nitride (h-BN) threshold memristors with two nickel (Ni) electrodes through their current conduction mechanisms. Both the high and the low resistance states are analyzed through temperature-dependent current-voltage measurements. We propose the formation and retraction of nickel filaments along boron defects in the h-BN film as the resistive switching mechanism. We corroborate our electrical data with TEM analyses to establish temperature-dependent current-voltage measurements as a valuable tool for the analysis of resistive switching phenomena in memristors made of 2D materials. Our memristors exhibit a wide and tunable current operation range and low stand-by currents, in line with the state of the art in h-BN-based threshold switches, a low cycle-to-cycle variability of 5%, and a large On/Off ratio of 10${^7}$.",2301.10158v2 2021-08-21,Resistivity size effect due to surface steps on ruthenium thin films computed with a realistic tight-binding model,"A realistic tight-binding model is developed and employed to elucidate the resistivity size effect due to steps on Ru thin films. The resistivity of two different film orientations, $(0001)$ and $(1 \bar{1}00)$, is computed for transport along a $[1 1 \bar{2} 0]$ direction both for smooth surfaces and for surfaces with monolayer-high steps. In the case of smooth films, the systems are also studied using solutions to the Boltzmann transport equation (BTE). Interestingly, the resistivity of $(1 \bar{1}00)$ surfaces exhibits a significant size effect even in the absence of surface steps. When monolayer-high steps are spaced $\sim 10$ nm apart, the resistivity is shown to increase due to scattering from the steps. However, only a small increase was found which cannot explain the large effect seen in recent experiments with Ru thin films. This highlights the need for further elucidation of the resistivity size effect. Theoretical analysis suggest that films made from materials with a relatively large ballistic conductance per area like Ru should exhibit a reduced resistivity size effect. This result points to Ru as a promising interconnect material. Finally, because a very efficient algorithm for computing resistivity based on the kernel polynomial method (KPM) is used, the approach fulfills a need for realistic models that can span length scales directly relevant to experimental results. The calculations described here include films approaching $5$ nm in thickness, with in-plane distances up to $\sim 160$ nm and $3.8\times10^{5}$ atomic sites.",2108.09424v7 2018-11-14,Linear-in-T resistivity in dilute metals: A Fermi liquid perspective,"We consider a short-range deformation potential scattering model of electron-acoustic phonon interaction to calculate the resistivity of an ideal metal as a function of temperature (T) and electron density (n). We consider both 3D metals and 2D metals, and focus on the dilute limit, i.e., low effective metallic carrier density of the system. The main findings are: (1) a phonon scattering induced linear-in-T resistivity could persist to arbitrarily low T in the dilute limit independent of the Debye temperature ($T_D$) although eventually the low-T resistivity turns over to the expected Bloch-Gruneisen (BG) behavior with $T^5$ ($T^4$) dependence, in 3D (2D) respectively; (2) because of low values of n, the phonon-induced resistivity could be very high in the system; (3) the resistivity shows an intrinsic saturation effect at very high temperatures (for $T>T_D$), and in fact, decreases with increasing T above a high crossover temperature with this crossover being dependent on both $T_D$ and n in a non-universal manner. We also provide high-T linear-in-T resistivity results for 2D and 3D Dirac materials. Our work brings out the universal features of phonon-induced transport in dilute metals, and we comment on possible implications of our results for strange metals, emphasizing that the mere observation of a linear-in-T metallic resistivity at low temperatures or a very high metallic resistivity at high temperatures is not necessarily a reason to invoke an underlying quantum critical strange metal behavior. We discuss the temperature variation of the effective transport scattering rate showing that the scattering rate could be below or above $k_BT$, and in particular, purely coincidentally, the calculated scattering rate happens to be $k_BT$ in normal metals with no implications for the so-called Planckian behavior.",1811.05862v2 2012-04-10,Challenges for RPCs and resistive micropattern detectors in the next few years,"Nowadays RPCs are in a booming phase: they are successfully used in many experiments, including LHC; there are ambitious plans to use them in several upgrade detectors and in some new experiments as well as in various applications. The aim of this paper is to highlight the main challenges which the RPC community may face in the next few years and which were addressed in talks presented at this conference. Examples could be: new and difficult requirements from experiments (and their upgrades) and applications, optimization and improvements of the existing traditional detector designs, improvement of their characteristics (timing /rate performance, aging, dark current and so on), implementation of new more sensitive electronics, investigation of new materials, development of large- area detectors. We will also review the fast and very promising developments of another type of resistive electrode gaseous detector -micropattern detectors having at least one of their electrodes made of resistive materials. These innovative detectors combine in one design the best features of RPC (spark protection) and micropattern detectors (high granularity-high position resolution).",1204.2144v1 2021-01-28,Magnetic Field Effects on the Transport Properties of High-Tc Cuprates,"Starting from a recently proposed comprehensive theory for the high-Tc superconductivity in cuprates, we derive a general analytic expression for the planar resistivity, in the presence of an applied external magnetic field $\textbf{H}$ and explore its consequences in the different phases of these materials. As an initial probe of our result, we show it compares very well with experimental data for the resistivity of LSCO at different values of the applied field. We also apply our result to Bi2201 and show that the magnetoresistivity in the strange metal phase of this material, exhibits the $H^2$ to $H$ crossover, as we move from the weak to the strong field regime. Yet, despite of that, the magnetoresistivity does not present a quadrature scaling. Remarkably, the resistivity H-field derivative does scale as a function of $\frac{H}{T}$, in complete agreement with recent magneto-transport measurements made in the strange metal phase of cuprates \cite{Hussey2020}. We, finally, address the issue of the $T$-power-law dependence of the resistivity of overdoped cuprates and compare our results with experimental data for Tl2201. We show that this provides a simple method to determine whether the quantum critical point associated to the pseudogap temperature $T^*(x)$ belongs to the SC dome or not.",2101.11969v1 2022-09-08,Dominance of Electron-Magnon Scattering in Itinerant Ferromagnet Fe3GeTe2,"Fe3GeTe2 is a 2-dimensional van der Waals material exhibiting itinerant ferromagnetism upto 230 K. Here, we study aspects of scattering mechanism in Fe3Ge2Te2 single crystals via resistivity, magneto-transport and Hall effect measurements. The quadratic temperature dependence of electrical resistivity below the Curie temperature hints towards the dominance of electron-magnon scattering. A non-saturating positive magnetoresistance (MR) is observed at low temperatures when the magnetic field is applied parallel to the sample plane. The linear negative MR at high fields for T < TC corroborates to the suppression in magnon population due to the damping of spin waves. In the high temperature regime T > TC,MR can be described by the scattering from spin fluctuations using the model described by Khosla and Fischer. Isothermal Hall resistivity curves unveil the presence of anomalous Hall resistivity. Correlation between MR and side jump mechanism further reveals that the electron-magnon scattering is responsible for the side jump contribution to the anomalous Hall effect. Our results provide a clear understanding of the role of electron-magnon scattering on anomalous Hall effect that rules out its origin to be the topological band structure.",2209.03555v1 2014-12-01,Novel experimental design for high pressure - high temperature electrical resistance measurements in a 'Paris-Edinburgh' large volume press,"We present a novel experimental design for high sensitivity measurements of the electrical resistance of samples at high pressures (0-6GPa) and high temperatures (300-1000K) in a 'Paris-Edinburgh' type large volume press. Uniquely, the electrical measurements are carried out directly on a small sample, thus greatly increasing the sensitivity of the measurement. The sensitivity to even minor changes in electrical resistance can be used to clearly identify phase transitions in material samples. Electrical resistance measurements are relatively simple and rapid to execute and the efficacy of the present experimental design is demonstrated by measuring the electrical resistance of Pb, Sn and Bi across a wide domain of temperature-pressure phase space and employing it to identify the loci of phase transitions. Based on these results, the phase diagrams of these elements are reconstructed to high accuracy and found to be in excellent agreement with previous studies. In particular, by mapping the locations of several well-studied reference points in the phase diagram of Sn and Bi, it is demonstrated that a standard calibration exists for the temperature and pressure, thus eliminating the need for direct or indirect temperature and pressure measurements. The present technique will allow simple and accurate mapping of phase diagrams under extreme conditions and may be of particular importance in advancing studies of liquid state anomalies.",1412.0613v2 2010-05-13,Gravitational-wave spin-down and stalling lower limits on the electrical resistivity of the accreted mountain in a millisecond pulsar,"The electrical resistivity of the accreted mountain in a millisecond pulsar is limited by the observed spin-down rate of binary radio millisecond pulsars (BRMSPs) and the spins and X-ray fluxes of accreting millisecond pulsars (AMSPs). We find $\eta \ge 10^{-28}\,\mathrm{s}\, (\tau_\mathrm{SD}/1\,\mathrm{Gyr})^{-0.8}$ (where $\tau_\mathrm{SD}$ is the spin-down age) for BRMSPs and $\eta \ge 10^{-25}\,\mathrm{s}\,(\dot{M}_\mathrm{a}/\dot{M}_\mathrm{E})^{0.6}$ (where $\dot{M}_\mathrm{a}$ and $\dot{M}_\mathrm{E}$ are the actual and Eddington accretion rates) for AMSPs. These limits are inferred assuming that the mountain attains a steady state, where matter diffuses resistively across magnetic flux surfaces but is replenished at an equal rate by infalling material. The mountain then relaxes further resistively after accretion ceases. The BRMSP spin-down limit approaches the theoretical electron-impurity resistivity at temperatures $\ga 10^5$ K for an impurity concentration of $\sim 0.1$, while the AMSP stalling limit falls two orders of magnitude below the theoretical electron-phonon resistivity for temperatures above $10^8$ K. Hence BRMSP observations are already challenging theoretical resistivity calculations in a useful way. Next-generation gravitational-wave interferometers will constrain $\eta$ at a level that will be competitive with electromagnetic observations.",1005.2257v1 2017-01-23,Crystal Growth and Magneto-transport of Bi2Se3 Single crystals,"In this letter, we report growth and characterization of bulk Bi2Se3 single crystals. The studied Bi2Se3 crystals are grown by self flux method through solid state reaction from high temperature (950C) melt of constituent elements and slow cooling (2C/hour). The resultant crystals are shiny and grown in [00l] direction, as evidenced from surface XRD. Detailed Reitveld analysis of PXRD (powder x-ray diffraction) of the crystals showed that these are crystallized in rhombohedral crystal structure with space group of R3m (D5) and the lattice parameters are a = 4.14(2)A, b = 4.14 (2) A and c = 28.7010(7) A. Temperature versus resistivity (R-T) plots revealed metallic conduction down to 2K, with typical room temperature resistivity (R300K) of around 0.53 mohm-cm and residual resistivity of 0.12 mohm-cm. Resistivity under magnetic field ] measurements exhibited large +Ve magneto resistance right from 2K to 200K. Isothermal magneto resistance [RH] measurements at 2K, 100K and 200K exhibited magneto resistance (MR) of up to 240, 130 and 60 percent respectively at 14 Tesla. Further the MR plots are non saturating and linear with field at all temperature. At 2K the MR plots showed clear quantum oscillations at above say 10 Tesla applied field. Also the Kohler plots i.e., were seen consolidating on one plot. Interestingly, the studied Bi2Se3 single crystal exhibited the Shubnikov-de Haas oscillations (SdH) at 2K under different applied magnetic fields ranging from 4Tesla to 14 Tesla",1701.06280v2 2020-06-24,Conductive filament evolution dynamics revealed by cryogenic (1.5 K) multilevel switching of CMOS-compatible Al2O3/TiO2 resistive memories,"This study demonstrates multilevel switching at 1.5 K of Al2O3/TiO2-x resistive memory devices fabricated with CMOS-compatible processes and materials. The I-V characteristics exhibit a negative differential resistance (NDR) effect due to a Joule-heating-induced metal-insulator transition of the Ti4O7 conductive filament. Carrier transport analysis of all multilevel switching I-V curves show that while the insulating regime follows the space charge limited current (SCLC) model for all resistance states, the conduction in the metallic regime is dominated by SCLC and trap-assisted tunneling (TAT) for low- and high-resistance states respectively. A non-monotonic conductance evolution is observed in the insulating regime, as opposed to the continuous and gradual conductance increase and decrease obtained in the metallic regime during the multilevel SET and RESET operations. Cryogenic transport analysis coupled to an analytical model accounting for the metal-insulator-transition-induced NDR effects and the resistance states of the device provide new insights on the conductive filament evolution dynamics and resistive switching mechanisms. Our findings suggest that the non-monotonic conductance evolution in the insulating regime is due to the combined effects of longitudinal and radial variations of the Ti4O7 conductive filament during the switching. This behavior results from the interplay between temperature- and field-dependent geometrical and physical characteristics of the filament.",2006.13394v1 2002-04-23,"Effects of stoichiometry, purity, etching and distilling on resistance of MgB2 pellets and wire segments","We present a study of the effects of non-stoichiometry, boron purity, wire diameter and post-synthesis treatment (etching and Mg distilling) on the temperature dependent resistance and resistivity of sintered MgB2 pellets and wire segments. Whereas the residual resistivity ratio (RRR) varies between RRR \~ 4 to RRR > 20 for different boron purity, it is only moderately affected by non-stoichiometry (from 20% Mg deficiency to 20% Mg excess) and is apparently independent of wire diameter and presence of Mg metal traces on the wire surface. The obtained set of data indicates that RRR values in excess of 20 and residual resistivities as low as rho{0} ~ 0.4 mu Ohm cm are intrinsic material properties of high purity MgB2.",0204510v1 2007-01-19,Resistance Anomaly in Disordered Superconducting Films,"We report on a resistance anomaly in disordered superconducting films containing arrays of irregularly distributed nanoscale holes. At high driving currents, peaks appear in the resistance as a function of temperature, with peak values up to 2% above the classic normal-state resistance. We attribute the observed resistance anomaly to dissipation-induced granularity which enhances the contributions from fluctuation-induced reduction of the density of states of the quasiparticles. The granular feature of a disordered superconducting film originates from the inhomogeneous temperature distribution caused by the variation of the local dissipation and/or heat transfer.",0701483v1 2007-07-28,Giant Magneto-impedance in stress-annealed Finemet/Copper/Finemet based trilayer structures,"The resistive and reactive components of magneto-impedance (MI) for Finemet/Copper/Finemet sandwiched structures based on stress-annealed nanocrystalline Fe75Si15B6Cu1Nb3 ribbons as functions of different fields (longitudinal and perpendicular) and frequencies have been measured and analyzed. Maximum magneto-resistance and magneto-inductance ratios of 700% and 450% have been obtained in 30-600 kHz frequency range respectively. These large magneto-resistance and magneto-inductive ratios are a direct consequence of the large effective relative permeability due to the closed magnetic flux path in the trilayer structure. The influence of perpendicular bias fields (Hper) in the Longitudinal Magneto-impedance (LMI) configuration greatly improves the MI ratios and sensitivities. The maximum MI ratio for the resistive part increases to as large as 2500% for Hper ~ 1 Oe. The sensitivity of the magneto-resistance increases from 48%/Oe to 288%/Oe at 600 kHz frequency with the application of Hper ~ 30 Oe. Such high increase in MI ratios and sensitivities with perpendicular bias fields are due to the formation the favourable (transverse) domain structures.",0707.4229v1 2010-04-12,Systematic Investigation of the Intrinsic Channel Properties and Contact Resistance of Monolayer and Multilayer Graphene FET,"The intrinsic channel properties of monolayer and multilayer graphene were systematically investigated as a function of layer number by the exclusion of contact resistance using four-probe measurements. We show that the continuous change in normalized sheet resistivity from graphite to a bilayer graphene is governed by one unique property, i.e., the band overlap, which markedly increases from 1 meV for a bilayer graphene to 11 meV for eight layers and eventually reaches 40 meV for graphite. The monolayer graphene, however, showed a deviation in temperature dependence due to a peculiar linear dispersion. Additionally, contact resistivity was extracted for the case of typical Cr/Au electrodes. The observed high contact resistivity, which varies by three orders of magnitude (from ~103 to 106 Ohm micron), might significantly mask the outstanding performance of the monolayer graphene channel, suggesting its importance in future research.",1004.2074v1 2010-09-02,Kondo and charge fluctuation resistivity due to Anderson impurities in graphene,"Motivated by experiments on ion irradiated graphene, we compute the resistivity of graphene with dilute impurities. In the local moment regime we employ the perturbation theory up to third order in the exchange coupling to determine the behavior at high temperatures within the Kondo model. Resistivity due to charge fluctuations is obtained within the mean field approach on the Anderson impurity model. Due to the linear spectrum of the graphene the Kondo behavior is shown to depend on the gate voltage applied. The location of the impurity on the graphene sheet is an important variable determining its effect on the Kondo scale and resistivity. Our results show that for chemical potential nearby the node the charge fluctuations is responsible for the observed temperature dependence of resistivity while away from the node the spin fluctuations take over. Quantitative agreement with experimental data is achieved if the energy of the impurity level varies linearly with the chemical potential.",1009.0551v3 2017-10-05,Electric field Control of Exchange Bias by Resistive Switching,"We demonstrated an electric field controlled exchange bias (EB) effect accompanied with unipolar resistive switching behavior in the Si/SiO2/Pt/Co/NiO/Pt device. By applying certain voltages, the device displays obvious EB in high-resistance-state while negligible EB in low-resistance-state. Conductive filaments forming and rupture in the NiO layer but near the Co-NiO interface are considered to play dominant roles in determining the combined resistive switching and EB phenomena. This work paves a new way for designing multifunctional and nonvolatile magnetic-electrical random access memory devices.",1710.01865v1 2018-06-11,Conductivity and Resistivity of Dirac Electrons in Single-Component Molecular Conductor [Pd(dddt)_2],"Dirac electrons, which have been found in the single-component molecular conductor [Pd(dddt)_2] under pressure, are examined by calculating the conductivity and resistivity in terms of a tight-binding model for several pressures of P GPa, which give a nodal line semimetal or insulator. The temperature (T) dependence of the conductivity shows that the conductivity increases linearly under pressure at low T due to the Dirac cone but stays almost constant at high T. Further, at lower pressures, the conductivity is suppressed due to an unconventional gap, which is examined by calculating the resistivity. The resistivity exhibits a pseudogap-like behavior even in the case described by the Dirac cone. Such behavior originates from a novel role of the nodal line semimetal followed by a pseudogap that is different from a band gap. The present result reasonably explains the resistivity observed in the experiment.",1806.03819v2 2019-05-29,Intrinsic resistance peaks in AB-stacked multilayer graphene with odd number of layers,"The intrinsic resistance peak (ridge) structures were recently found to appear in the carrier density dependence plot of the resistance of the AB-stacked multilayer graphene with even numbers of layers.The ridges are due to topological changes in the Fermi surface. Here, these structures were studied in AB-stacked multilayer graphene with odd numbers of layers (5 and 7 layers) by performing experiments using encapsulated high-quality graphene samples equipped with top and bottom gate electrodes.The intrinsic resistance peaks that appeared on maps plotted with respect to the carrier density and perpendicular electric field showed particular patterns depending on graphene's crystallographic structure, and were qualitatively different from those of graphene with even numbers of layers. Numerical calculations of the dispersion relation and semi-classical resistivity using information based on the Landau level structure determined by the magnetoresistance oscillations, revealed that the difference stemmed from the even-odd layer number effect on the electronic band structure.",1905.12193v2 2014-08-01,Resistive switching in ultra-thin La0.7Sr0.3MnO3 / SrRuO3 superlattices,"Superlattices may play an important role in next generation electronic and spintronic devices if the key-challenge of the reading and writing data can be solved. This challenge emerges from the coupling of low dimensional individual layers with macroscopic world. Here we report the study of the resistive switching characteristics of a of hybrid structure made out of a superlattice with ultrathin layers of two ferromagnetic metallic oxides, La0.7Sr0.3MnO3 (LSMO) and SrRuO3 (SRO). Bipolar resistive switching memory effects are measured on these LSMO/SRO superlattices, and the observed switching is explainable by ohmic and space charge-limited conduction laws. It is evident from the endurance characteristics that the on/off memory window of the cell is greater than 14, which indicates that this cell can reliably distinguish the stored information between high and low resistance states. The findings may pave a way to the construction of devices based on nonvolatile resistive memory effects.",1408.0103v1 2019-07-19,Niobium nitride thin films for very low temperature resistive thermometry,"We investigate thin film resistive thermometry based on metal-to-insulator-transition (niobium nitride) materials down to very low temperature. The variation of the NbN thermometer resistance have been calibrated versus temperature and magnetic field. High sensitivity in tempertaure variation detection is demonstrated through efficient temperature coefficient of resistance. The nitrogen content of the niobium nitride thin films can be tuned to adjust the optimal working temperature range. In the present experiment, we show the versatility of the NbN thin film technology through applications in very different low temperature use-cases. We demonstrate that thin film resistive thermometry can be extended to temperatures below 30 mK with low electrical impedance.",1907.08443v1 2018-07-23,Coexistence of Diamagnetism and Vanishingly Small Electrical Resistance at Ambient Temperature and Pressure in Nanostructures,"The great practical utility has motivated extensive efforts to discover ultra-low resistance electrical conductors and superconductors in ambience. Here we report the observation of vanishingly small electrical resistance at the ambient temperature and pressure conditions in films and pellets of a nanostructured material that is composed of silver particles embedded into a gold matrix. Upon cooling below a sample-specific temperature scale ($T_{C}$) as high as $286$ K, the film resistance drops below $\sim 2\mu\Omega$, being limited by measurement uncertainty. The corresponding resistivity ($\sim 10^{-12}$ $\Omega$.m) is at least four orders of magnitude below that of elemental noble metals, such as gold, silver or copper. Furthermore, the samples become strongly diamagnetic below $T_{C}$, with volume susceptibilities as low as -0.056. We additionally describe methods to tune $T_{C}$ to temperatures much higher than room temperature.",1807.08572v3 2022-11-22,Contact Resistance Study of Various Metal Electrodes with CVD Graphene,"In this study, the contact resistance of various metals to chemical vapour deposited (CVD) monolayer graphene is investigated. Transfer length method (TLM) structures with varying widths and separation between contacts have been fabricated and electrically characterized in ambient air and vacuum condition. Electrical contacts are made with five metals: gold, nickel, nickel/gold, palladium and platinum/gold. The lowest value of 92 {\Omega}{\mu}m is observed for the contact resistance between graphene and gold, extracted from back-gated devices at an applied back-gate bias of -40 V. Measurements carried out under vacuum show larger contact resistance values when compared with measurements carried out in ambient conditions. Post processing annealing at 450{\deg}C for 1 hour in argon-95% / hydrogen-5% atmosphere results in lowering the contact resistance value which is attributed to the enhancement of the adhesion between metal and graphene. The results presented in this work provide an overview for potential contact engineering for high performance graphene-based electronic devices.",2211.12415v1 2023-03-06,Quantum Acoustics Spawns Planckian Resistivity,"Strange metals exhibit universal linear-in-temperature resistivity described by a Planckian scattering rate, the origin of which remains elusive. By employing a novel approach inspired by quantum optics, we arrive at the coherent state limit of lattice vibrations: quantum acoustics. Utilizing this nonperturbative framework, we demonstrate that lattice vibrations are active drivers in the Planckian resistivity phenomenon, challenging prevailing theories. Treating charge carriers as quantum wave packets negotiating the dynamic acoustic field, competition ensues between localization and delocalization, settling on the conjectured universal quantum bound of diffusion and capturing the enigmatic $T$-linear resistivity over hundreds of degrees. Our research not only elucidates the critical role of phonons in Planckian resistivity but also redefines their significance in the broader landscape of high-temperature superconductivity and condensed matter physics.",2303.06077v3 2011-04-11,DOS-limited contact resistance in graphene FETs,"Graphene has attracted much attention as one of promising candidates of future high-speed transistor materials because of its high carrier mobility of more than 10,000 cm2 V-1 s-1. Up to this point, we have focused on the contact properties as performance killers, as a very small density of states in graphene might suppress the current injection from metal to graphene. This paper systematically reviews the metal/graphene contact properties and discusses the present status and future requirements of the specific contact resistivity.",1104.1818v1 2006-07-28,Contact effects in polymer field-effect transistors,"Contact resistances often contribute significantly to the overall device resistance in organic field-effect transistors (OFETs). Understanding charge injection at the metal-organic interface is critical to optimizing OFET device performance. We have performed a series of experiments using bottom-contact poly(3-hexylthiophene) (P3HT) OFETs in the shallow channel limit to examine the injection process. When contacts are ohmic we find that contact resistivity is inversely proportional to carrier mobility, consistent with diffusion-limited injection. However, data from devices with other electrode materials indicate that this simple picture is inadequate to describe contacts with significant barriers. A generalized transmission line method allows the analysis of nonohmic contacts, and we find reasonable agreement with a model for injection that accounts for the hopping nature of conduction in the polymer. Variation of the (unintentional) dopant concentration in the P3HT can significantly alter the injection process via changes in metal-organic band alignment. At very low doping levels, transport suggests the formation of a barrier at the Au/P3HT interface, while Pt/P3HT contacts remain ohmic with comparatively low resistance. We recently observed that self-assembled monolayers on the metal source/drain electrodes can significantly decrease contact resistance and maintain ohmic conduction under conditions that would result in nonohmic, high resistance contacts to untreated electrodes. Finally, we discuss measurements on extremely short channel devices, in the initial steps toward examining transport through individual polymer chains.",0607744v1 2008-11-21,Tuning the Correlation Decay in the Resistance Fluctuations of Multi-Species Networks,"A new network model is proposed to describe the $1/f^\alpha$ resistance noise in disordered materials for a wide range of $\alpha$ values ($0< \alpha < 2$). More precisely, we have considered the resistance fluctuations of a thin resistor with granular structure in different stationary states: from nearly equilibrium up to far from equilibrium conditions. This system has been modelled as a network made by different species of resistors, distinguished by their resistances, temperature coefficients and by the energies associated with thermally activated processes of breaking and recovery. The correlation behavior of the resistance fluctuations is analyzed as a function of the temperature and applied current, in both the frequency and time domains. For the noise frequency exponent, the model provides $0< \alpha < 1$ at low currents, in the Ohmic regime, with $\alpha$ decreasing inversely with the temperature, and $1< \alpha <2$ at high currents, in the non-Ohmic regime. Since the threshold current associated with the onset of nonlinearity also depends on the temperature, the proposed model qualitatively accounts for the complicate behavior of $\alpha$ versus temperature and current observed in many experiments. Correspondingly, in the time domain, the auto-correlation function of the resistance fluctuations displays a variety of behaviors which are tuned by the external conditions.",0811.3565v2 2023-07-01,"The near room-temperature upsurge of electrical resistivity in Lu-H-N is not superconductivity, but a metal-to-poor-conductor transition","Since the discovery of superconductivity in mercury at 4 K in 1911, searching for materials with superconductivity at higher temperatures towards practical conditions has been a primary enduring goal. The recent report of room-temperature superconductivity at near-ambient pressure in nitrogen-doped lutetium hydride (Lu-H-N) by Dasenbrock-Gammon et al. (Hereafter referred as D-G) seems a great step approaching the ultimate goal. Specifically, they claimed evidence of superconductivity on Lu-H-N with a maximum Tc of 294 K at 1 GPa. However, the failure to observe the drastic temperature-dependent resistance change above 200 K in high-pressure synthesized Lu-H-N compounds, a prerequisite for superconductivity, by researchers worldwide in all independent follow-up studies casts a heavy shadow on the authenticity of the claims. The sober questions are: what is the sample that produces the sharp resistance jump near room temperature? What are the reasons for the non-reproducibility of others who follow the D-G method of synthesis and the inscrutable low success rate (35%) in synthesizing the right sample even for the authors in Ref. 1? What causes the observed sharp resistance jump? Here, with a well-controlled experiment protocol, we repeatedly reproduced the near room-temperature sudden change of electrical resistance in the Lu-H-N sample, and we could quantitatively compare its behavior with the initial pure Lu in a normal metallic state. These results enable us to scrutinize the origin for the near-room temperature sharp resistance change, which is attributed to a metal-to-poor-conductor transition rather than superconductivity.",2307.00201v1 2020-01-17,"Magnetic, magnetoelastic and corrosion resistant properties of (Fe-Ni) based metallic glasses for structural health monitoring applications","We have performed a study of the magnetic, magnetoelastic, and corrosion resistance properties of seven different composition magnetoelastic-resonant platforms. For some applications, such as structural health monitoring, these materials must have not only good magnetomechanical properties, but also a high corrosion resistance. In the fabricated metallic glasses of composition Fe(73-x)NixCr5Si10B12, the Fe/Ni ratio was varied (Fe + Ni = 73% at.) thus changing the magnetic and magnetoelastic properties. A small amount of chromium (Cr5) was added in order to achieve the desired good corrosion resistance. As expected, all the studied properties change with the composition of the samples. Alloys containing a higher amount of Ni than Fe do not show magnetic behavior at room temperature, while iron-rich alloys have demonstrated not only good magnetic properties, but also good magnetoelastic ones, with magnetoelastic coupling coefficient as high as 0.41 for x=0 in the Fe73Ni0Cr5Si10B12 (the sample containing only Fe but not Ni). Concerning corrosion resistance, we have found a continuous degradation of these properties as the Ni content increases in the composition. Thus, the corrosion potential decreases monotonously from 46.74 mV for the x=0 composition, Fe73Ni0Cr5Si10B12 to -239.47 mV for the x=73 composition Fe0Ni73Cr5Si10B12.",2001.06283v1 2014-05-08,Controlling boron redistribution in CoFeB/MgO magnetic tunnel junctions during annealing by variation of cap layer materials and MgO deposition methods,"Magnetic tunnel junctions with crystalline MgO tunnel barrier and amorphous CoFeB electrodes received much attention due to their high tunnel magneto resistance ratio at room temperature. One important parameter for achieving high tunnel magneto resistance ratios is to control the boron diffusion from the electrodes especially during post growth annealing. By high resolution transmission electron microscopy and electron energy loss spectroscopy techniques we show that the cap layer material adjacent to the electrodes and the MgO deposition method are crucial to control boron redistribution. It is pointed out, that Ta cap layers acts as sinks for boron during annealing in contrast to Ru layers. Furthermore, radio frequency sputtered MgO tunneling barriers contain a rather high concentraion of boron in trigonal [BO$_3$]$^{3-}$ - environment after annealing in contrast to electron beam evaporated MgO which is virtually free from any boron. Our data further indicate that neither boron nor oxygen-vacancy-related gap states in the bulk of MgO barriers affect spin polarized transport for tunnel magneto resistance ratios at the level of 200%.",1405.1907v1 2021-10-20,Materials and possible mechanisms of extremely large magnetoresistance: A review,"Magnetoresistance (MR) is a characteristic that the resistance of a substance changes with the external magnetic field, reflecting various physical origins and microstructures of the substance. A large MR, namely a huge response to a low external field, has always been a useful functional feature in industrial technology and a core goal pursued by physicists and materials scientists. Conventional large MR materials are mainly manganites, whose colossal MR (CMR) can be as high as -90%. The dominant mechanism is attributed to spin configuration aligned by the external field, which reduces magnetic scattering and thus resistance. In recent years, some new systems have shown an extremely large unsaturated MR (XMR). Unlike ordinary metals, the positive MR of these systems can reach 103-108% and is persistent under super high magnetic fields. The XMR materials are mainly metals or semimetals, distributed in high-mobility topological or non-topological systems, and some are magnetic, which suggests a wide range of application scenarios. Various mechanisms have been proposed for the potential physical origin of XMR, including electron-hole compensation, steep band, ultrahigh mobility, high residual resistance ratio, topological fermions, etc. It turns out that some mechanisms play a leading role in certain systems, while more are far from clearly defined. In addition, the researches on XMR are largely overlapped or closely correlated with other recently rising physics and materials researches, such as topological matters and two-dimensional (2D) materials, which makes elucidating the mechanism of XMR even more important. Moreover, the disclosed novel properties will lay a broad and solid foundation for the design and development of functional devices. In this review, we will discuss several aspects in the following order: ...",2110.10454v1 2024-05-09,Extreme high lattice-misfit superalloys with regular cubic L12 particles and excellent creep resistance,"In novel Co and CoNi based superalloys, the creep resistance is limited at high temperatures due to low lattice misfit and solvus temperature. In this study, we combined the advantages of Co-Ti (high lattice misfit and solvus temperature) and Co-Al based superalloys (cuboidal precipitates) by using Ti to substitute Al in alloys of Co-30Ni-(12.5-x)Al-xTi-2.5Mo-2.5W (at.%) composition. With high Ti content, the alloys obtained extreme high lattice misfit (bigger than 1.3 %) and solvus temperature (bigger than 1150 degree). During aging at 900 degree, alloys with high Ti/Al ratio exhibited a lower gamma prime precipitate coarsening rate resulting from their lower gamma prime and gamma interfacial energy and higher lattice misfit. In addition, high Ti/Al ratio brought higher gamma prime volume fraction and excellent mechanical properties, such as higher yield stress and better creep resistance. However, at high temperature of 1100 degree, the cubic gamma prime phase was decomposed into deleterious Eta phase with D024 structure if the Ti/Al ratio exceeded 1. Based on this, we outreached new alloys design with a high content of Cr and Ta and appropriate Ti/Al ratio, i.e., Ti/Al ratio is smaller than 1. The newly designed alloys still have high solvus temperature (bigger than 1200 degree) and exhibit high lattice misfit (bigger than 1.2 %) as Co-12Ti (at.%) superalloys but more regular cubic gamma prime precipitates and significantly better creep resistance than superalloys Co-9Al-9W and Co-9Al-9W-2Ti at 850 and 950 degree. Nevertheless, compared with creep resistance of Ni based superalloys, our newly designed alloys still need to be further improved, especially in the 1000 and 1050 degree range.",2405.05851v1 2019-01-28,Strong damping-like spin-orbit torque and tunable Dzyaloshinskii-Moriya interaction generated by low-resistivity Pd$_{1-x}$Pt$_x$ alloys,"Despite their great promise for providing a pathway for very efficient and fast manipulation of magnetization at the nanoscale, spin-orbit torque (SOT) operations are currently energy inefficient due to a low damping-like SOT efficiency per unit current bias, and/or the very high resistivity of the spin Hall materials. Here, we report an advantageous spin Hall material, Pd1-xPtx, which combines a low resistivity with a giant spin Hall effect as evidenced through the use of three independent SOT ferromagnetic detectors. The optimal Pd0.25Pt0.75 alloy has a giant internal spin Hall ratio of >0.47 (damping-like SOT efficiency of ~ 0.26 for all three ferromagnets) and a low resistivity of ~57.5 {\mu}{\Omega} cm at 4 nm thickness. Moreover, we find the Dzyaloshinskii-Moriya interaction (DMI), the key ingredient for the manipulation of chiral spin arrangements (e.g. magnetic skyrmions and chiral domain walls), is considerably strong at the Pd1-xPtx/Fe0.6Co0.2B0.2 interface when compared to that at Ta/Fe0.6Co0.2B0.2 or W/Fe0.6Co0.2B0.2 interfaces and can be tuned by a factor of 5 through control of the interfacial spin-orbital coupling via the heavy metal composition. This work establishes a very effective spin current generator that combines a notably high energy efficiency with a very strong and tunable DMI for advanced chiral spintronics and spin torque applications.",1901.09954v1 2014-10-29,Contact Research Strategy for Emerging Molybdenum Disulfide and Other Two-Dimensional Field-effect Transistors,"Layered two-dimensional (2D) semiconducting transition metal dichalcogenides (TMD) have been widely isolated, synthesized, and characterized recently. Numerous 2D materials are identified as the potential candidates as channel materials for future thin film technology due to their high mobility and the exhibiting bandgaps. While many TMD filed-effect transistors (FETs) have been widely demonstrated along with a significant progress to clearly understand the device physics, large contact resistance at metal/semiconductor interface still remain a challenge. From 2D device research point of view, how to minimize the Schottky barrier effects on contacts thus reduce the contact resistance of metals on 2D materials is very critical for the further development of the field. Here, we present a review of contact research on molybdenum disulfide and other TMD FETs from the fundamental understanding of metal-semiconductor interfaces on 2D materials. A clear contact research strategy on 2D semiconducting materials is developed for future high-performance 2D FETs with aggressively scaled dimensions.",1410.8201v1 2023-06-29,Speeding up high-throughput characterization of materials libraries by active learning: autonomous electrical resistance measurements,"High-throughput experimentation enables efficient search space exploration for the discovery and optimization of new materials. However, large search spaces of, e.g., compositionally complex materials, require decreasing characterization times significantly. Here, an autonomous measurement algorithm was developed, which leverages active learning based on a Gaussian process model capable of iteratively scanning a materials library based on the highest uncertainty. The algorithm is applied to a four-point probe electrical resistance measurement device, frequently used to obtain indications for regions of interest in materials libraries. Ten materials libraries with different complexities of composition and property trends are analyzed to validate the model. By stopping the process before the entire library is characterized and predicting the remaining measurement areas, the measurement efficiency can be improved drastically. As robustness is essential for autonomous measurements, intrinsic outlier handling is built into the model and a dynamic stopping criterion based on the mean predicted covariance is proposed. A measurement time reduction of about 70-90% was observed while still ensuring an accuracy of above 90%.",2306.17277v1 2013-03-29,An operational window for radiation-resistant materials based on sequentially healing grain interiors and boundaries,"Design of nuclear materials with high radiation-tolerance has great significance1, especially for the next generation of nuclear energy systems2,3. Response of nano- and poly-crystals to irradiation depends on the radiation temperature, dose-rate and grain size4-13. However the dependencies had been studied and interpreted individually, and thus severely lacking is the ability to predict radiation performance of materials in extreme environments. Here we propose an operational window for radiation-resistant materials, which is based on a perspective of interactions among irradiation-induced interstitials, vacancies, and grain boundaries. Using atomic simulations, we find that healing grain boundaries needs much longer time than healing grain interiors. Not been noticed before, this finding suggests priority should be thereafter given to recovery of the grain boundary itself. This large disparity in healing time is reflected in the spectra of defects-recombination energy barriers by the presence of one high-barrier peak in addition to the peak of low barriers. The insight gained from the study instigates new avenues for examining the role of grain boundaries in healing the material. In particular, we sketch out the radiation-endurance window in the parameter space of temperature, dose-rate and grain size. The window helps evaluate material performance and develop resistant materials against radiation damage.",1303.7316v1 2004-09-08,Magnetic and electronic phase transformations in (Sm0.65Sr0.35)MnO3 induced by temperature and magnetic field,"Temperature (4.2-260 K) and magnetic field (0-50 kOe) dependencies of the dc electrical resistance, dc magnetization, and ac magnetic susceptibility of (Sm0.65Sr0.35)MnO3 prepared from high purity components have been studied.",0409213v1 2015-11-19,High performance sensors based on resistance fluctuations of single layer graphene transistors,"One of the most interesting predicted applications of graphene monolayer based devices is as high quality sensors. In this letter we show, through systematic experiments, a chemical vapor sensor based on the measurement of low frequency resistance fluctuations of single layer graphene field-effect-transistor (SLG-FET) devices. The sensor has extremely high sensitivity, very high specificity, high fidelity and fast response times. The performance of the device using this scheme of measurement (which uses resistance fluctuations as the detection parameter) is more than two orders of magnitude better than a detection scheme where changes in the average value of the resistance is monitored. We propose a number-density fluctuation based model to explain the superior characteristics of noise measurement based detection scheme presented in this article.",1511.06213v1 2014-08-19,Aluminium-oxide wires for superconducting high kinetic inductance circuits,"We investigate thin films of conducting aluminium-oxide, also known as granular aluminium, as a material for superconducting high quality, high kinetic inductance circuits. The films are deposited by an optimised reactive DC magnetron sputter process and characterised using microwave measurement techniques at milli-Kelvin temperatures. We show that, by precise control of the reactive sputter conditions, a high room temperature sheet resistance and therefore high kinetic inductance at low temperatures can be obtained. For a coplanar waveguide resonator with 1.5\,k$\Omega$ sheet resistance and a kinetic inductance fraction close to unity, we measure a quality factor in the order of 700\,000 at 20\,mK. Furthermore, we observe a sheet resistance reduction by gentle heat treatment in air. This behaviour is exploited to study the kinetic inductance change using the microwave response of a coplanar wave guide resonator. We find the correlation between the kinetic inductance and the sheet resistance to be in good agreement with theoretical expectations.",1408.4347v3 2013-05-05,Resistance of High-Temperature Cuprate Superconductors,"Cuprate superconductors have many different atoms per unit cell. A large fraction of cells (5-25%) must be modified (""doped"") before the material superconducts. Thus it is not surprising that there is little consensus on the superconducting mechanism, despite almost 200,000 papers. Most astonishing is that for the simplest electrical property, the resistance, ""despite sustained theoretical efforts over the past two decades, its origin and its relation to the superconducting mechanism remain a profound, unsolved mystery."" Currently, model parameters used to fit normal state properties are experiment specific and vary arbitrarily from one doping to the other. Here, we provide a quantitative explanation for the temperature and doping dependence of the resistivity, Hall effect, and magnetoresistance in one self-consistent model by showing that cuprates are intrinsically inhomogeneous with a percolating metallic region and insulating regions. Using simple counting of dopant-induced plaquettes, we show that the superconducting pairing and resistivity are due to phonons.",1305.1058v1 2013-12-18,Cyclic electric field stress on bipolar resistive switching devices,"We have studied the effects of accumulating cyclic electrical pulses of increasing amplitude on the non-volatile resistance state of interfaces made by sputtering a metal (Au, Pt) on top of the surface of a cuprate superconductor YBa$_2$Cu$_3$O$_{7-\delta}$ (YBCO). We have analyzed the influence of the number of applied pulses $N$ on the relative amplitude of the remnant resistance change between the high ($R_H$) and the low ($R_L$) state [$\alpha=(R_{H}-R_{L})/R_{L}$] at different temperatures ($T$). We show that the critical voltage ($V_c$) needed to produce a resistive switching (RS, i.e. $\alpha >0$) decreases with increasing $N$ or $T$. We also find a power law relation between the voltage of the pulses and the number of pulses $N_{\alpha_0}$ required to produce a RS of $\alpha=\alpha_0$. This relation remains very similar to the Basquin equation used to describe the stress-fatigue lifetime curves in mechanical tests. This points out to the similarity between the physics of the RS, associated with the diffusion of oxygen vacancies induced by electrical pulses, and the propagation of defects in materials subjected to repeated mechanical stress.",1312.5338v1 2014-06-13,Subcoercive and multilevel ferroelastic remnant states with resistive readout,"Ferroelectric devices use their electric polarization ferroic order as the switching and storage physical quantity for memory applications. However, additional built-in physical quantities and memory paradigms are requested for applications. We propose here to take advantage of the multiferroic properties of ferroelectrics, using ferroelasticity to create a remnant strain, persisting after stressing the material by converse piezoelectricity means. While large electric fields are needed to switch the polarization, here writing occurs at subcoercive much lower field values, which can efficiently imprint multiple remnant strain states. A proof-of-principle device, with the simplest and non-optimized resistance strain detection design, is shown here to exhibit 13-memory states of high reproducibility and reliability. The related advantages in lower power consumption and limited device fatigue make our approach relevant for applications.",1406.3457v1 2023-03-08,Encoding multistate charge order and chirality in endotaxial heterostructures,"High-density phase change memory (PCM) storage is proposed for materials with multiple intermediate resistance states, which have been observed in 1$T$-TaS$_2$ due to charge density wave (CDW) phase transitions. However, the metastability responsible for this behavior makes the presence of multistate switching unpredictable in TaS$_2$ devices. Here, we demonstrate the fabrication of nanothick verti-lateral $H$-TaS$_2$/1$T$-TaS$_2$ heterostructures in which the number of endotaxial metallic $H$-TaS$_2$ monolayers dictates the number of resistance transitions in 1$T$-TaS$_2$ lamellae near room temperature. Further, we also observe optically active heterochirality in the CDW superlattice structure, which is modulated in concert with the resistivity steps, and we show how strain engineering can be used to nucleate these polytype conversions. This work positions the principle of endotaxial heterostructures as a promising conceptual framework for reliable, non-volatile, and multi-level switching of structure, chirality, and resistance.",2303.04387v3 2021-05-13,Interaction Effects and Viscous Magneto-Transport in a Strongly Correlated 2D Hole System,"Fermi liquid theory has been a foundation in understanding the electronic properties of materials. For weakly interacting two-dimensional (2D) electron or hole systems, electron-electron interactions are known to introduce quantum corrections to the Drude conductivity in the FL theory, giving rise to temperature dependent conductivity and magneto-resistance. Here we study the magneto-transport in a strongly interacting 2D hole system over a broad range of temperatures ($T$ = 0.09 to $>$1K) and densities $p=1.98-0.99\times10^{10}$ cm$^{-2}$ where the ratio between Coulomb energy and Fermi energy $r_s$ = 20 - 30. We show that while the system exhibits a negative parabolic magneto-resistance at low temperatures ($\lesssim$ 0.4K) characteristic of an interacting FL, the FL interaction corrections represent an insignificant fraction of the total conductivity. Surprisingly, a positive magneto-resistance emerges at high temperatures and grows with increasing temperature even in the regime $T \sim E_F$, close to the Fermi temperature. This unusual positive magneto-resistance at high temperatures is attributed to the collective viscous transport of 2D hole fluid in the hydrodynamic regime where holes scatter frequently with each other. These findings highlight the collective transport in a strongly interacting 2D system in the $r_s\gg 1$ regime and the hydrodynamic transport induced magneto-resistance opens up possibilities to new routes of magneto-resistance at high temperatures.",2105.06502v1 2015-04-29,Gate-Tunable Tunneling Resistance in Graphene/Topological Insulator Vertical Junctions,"Graphene-based vertical heterostructures, particularly stacks incorporated with other layered materials, are promising for nanoelectronics. The stacking of two model Dirac materials, graphene and topological insulator, can considerably enlarge the family of van der Waals heterostructures. Despite well understanding of the two individual materials, the electron transport properties of a combined vertical heterojunction are still unknown. Here we show the experimental realization of a vertical heterojunction between Bi2Se3 nanoplate and monolayer graphene. At low temperatures, the electron transport through the vertical heterojunction is dominated by the tunneling process, which can be effectively tuned by gate voltage to alter the density of states near the Fermi surface. In the presence of a magnetic field, quantum oscillations are observed due to the quantized Landau levels in both graphene and the two-dimensional surface states of Bi2Se3. Furthermore, we observe an exotic gate-tunable tunneling resistance under high magnetic field, which displays resistance maxima when the underlying graphene becomes a quantum Hall insulator.",1504.07780v3 2022-03-31,Towards automated design of corrosion resistant alloy coatings with an autonomous scanning droplet cell,"We present an autonomous scanning droplet cell platform designed for on-demand alloy electrodeposition and real-time electrochemical characterization for investigating the corrosion-resistance properties of multicomponent alloys. Automation and machine learning are currently driving rapid innovation in high throughput and autonomous materials design and discovery. We present two alloy design case studies: one focusing on a multi-objective corrosion resistant alloy optimization, and a case study highlighting the complexity of the multimodal characterization needed to provide insight into the underlying structural and chemical factors that drive observed material behavior. This motivates a close coupling between autonomous research platforms and scientific machine learning methodology that blends mechanistic physical models and black box machine learning models. This emerging research area presents new opportunities to accelerate materials synthesis, evaluation, and hence discovery and design.",2203.17049v1 2019-06-10,Quantum oscillation of thermal conductivity and violation of Weidemann-Franz law in TaAs$_2$ and NbAs$_2$,"We report a study of thermal conductivity and resistivity at ultra-low temperatures and in high magnetic fields for semi-metal materials TaAs$_2$ and NbAs$_2$ by using single crystal samples. The thermal conductivity is strongly suppressed in magnetic fields, having good correspondence with the large positive magnetoresistance, which indicates a dominant electronic contribution to thermal conductivity. In addition, not only the resistivity but also the thermal conductivity display clear quantum oscillations behavior at subKelvin temperatures and in magnetic fields up to 14 T. The most striking phenomenon is that the thermal conductivity show a $T^4$ behavior at very low temperatures, while the resistivity show a $T$-independent behavior. This indicates a strong violation of the Weidemann-Franz law and points to a non-Feimi liquid state of these materials.",1906.03961v3 2022-01-09,Resistivity testing of palladium dilution limits in CoPd alloys for hydrogen storage,"Palladium satisfies most of the requirements for an effective hydrogen storage material with two major drawbacks: it has a relatively low gravimetric hydrogen density and is prohibitively expensive for large-scale applications. Pd-based alloys should be considered as possible alternatives to a pure Pd. The question is how much one can dilute the Pd concentration in a variety of candidate materials while preserving hydrogen absorption capability. We demonstrate that the resistivity measurements of thin-film alloy samples can be used for a qualitative high-throughput screening and study of the hydrogen-absorbing properties over the entire range of palladium concentrations. Contrary to palladium-rich alloys where additional hydrogen scattering indicates a degree of hydrogen content, the diluted alloy films respond by a decrease of resistance due to their thickness expansion. Evidence of significant hydrogen absorption was found in thin CoPd films diluted to just 20% of Pd.",2201.02974v1 2023-05-26,Ferroelectricity driven-resistive switching and Schottky barrier modulation at CoPt/MgZnO interface for non-volatile memories,"Ferroelectric memristors have attracted much attention as a type of nonvolatile resistance switching memories in neuromorphic computing, image recognition, and information storage. Their resistance switching mechanisms have been studied several times in perovskite and complicated materials systems. It was interpreted as the modulation of carrier transport by polarization control over Schottky barriers. Here, we experimentally report the isothermal resistive switching across a CoPt/MgZnO Schottky barrier using a simple binary semiconductor. The crystal and texture properties showed high-quality and single-crystal Co$_{0.30}$Pt$_{0.70}$/Mg$_{0.20}$Zn$_{0.80}$O hetero-junctions. The resistive switching was examined by an electric-field cooling method that exhibited a ferroelectric T$_C$ of MgZnO close to the bulk value. The resistive switching across CoPt/MgZnO Schottky barrier was accompanied by a change in the Schottky barrier height of 26.5 meV due to an interfacial charge increase and/or orbital hybridization induced reversal of MgZnO polarization. The magnitude of the reversed polarization was estimated to be a reasonable value of 3.0 (8.25) $\mu$ C/cm$^2$ at 300 K (2 K). These findings demonstrated the utilities of CoPt/MgZnO interface as a potential candidate for ferroelectric memristors and can be extended to probe the resistive switching of other hexagonal ferroelectric materials.",2305.16563v3 2016-08-04,Bulk Superconductivity Induced by In-plane Chemical Pressure Effect in Eu0.5La0.5FBiS2-xSex,"We have investigated Se substitution effect to superconductivity of an optimally-doped BiS2-based superconductor Eu0.5La0.5FBiS2. Eu0.5La0.5FBiS2-xSex samples with x = 0-1 were synthesized. With increasing x, in-plane chemical pressure is enhanced. For x = 0.6, 0.8, and 1, superconducting transitions with a large shielding volume fraction are observed in magnetic susceptibility measurements, and the highest Tc is 3.8 K for x = 0.8. From low-temperature electrical resistivity measurements, a zero-resistivity state is observed for all the samples, and the highest Tc is observed for x = 0.8. With increasing Se concentration, characteristics of electrical resistivity changes from semiconducting-like to metallic, suggesting that the emergence of bulk superconductivity is linked with the enhanced metallicity. A superconductivity phase diagram of the Eu0.5La0.5FBiS2-xSex superconductor is established. Temperature dependences of electrical resistivity show an anomalous two-step transition under high magnetic fields. Hence, the resistivity data are analyzed with assuming in-plane anisotropy of upper critical field.",1608.01470v2 2018-11-03,Carbon nanotube/metal corrosion issues for nanotube coatings and inclusions in a matrix,"Corrosion is an inevitable phenomenon that is inherent in metals and even though there has been significant research on this subject, no ideal protection has been discovered to fully prevent corrosion. However, methods such as using protective coatings, and modifying the structure or composition of the material have been used to slow down gradual corrosion and fortunately they proved to be quite beneficial. The research focus has shifted to integrating novel materials and structures to improve the corrosion resistance of composites. Carbon nanotubes (CNTs) are an attractive and promising filler due to their chemical inertness and high mechanical, electrical, and thermal properties. CNTs can fill the gaps of metals and polymer-based composites by forming a passive layer on metals and promoting sacrificial protection in zinc rich polymer (ZRP) coatings, and can therefore function as an anti-corrosion filler. This paper reviews the research that has been performed to better understand the influence of CNTs on corrosion resistance in composites. Accordingly, in metal matrix composites (MMCs), most of the work has been carried out on electrodeposited coatings, namely Ni-based-CNT composites, which show improved corrosion resistance by CNT addition. On the other hand, there are a few papers that have studied the corrosion resistance of Mg-based-CNT composites and their corrosion results contradict those obtained from other metal-CNT composites. For ZRPs or polymer-based coatings there are a few papers that studied the effect of CNTs on the corrosion of said composites. It is believed that CNTs can strengthen the adhesion between the coating and the substrate and facilitate sacrificial protection by Zn particles by forming a conductive network, hence the improved corrosion resistance.",1812.03815v1 1997-04-29,Normal state c-axis resistivity of high T_c cuprate superconductors,"It is shown that a strong intraplanar incoherent scattering can effectively block the interplanar coherent tunneling between the weakly coupled planes of the highly anisotropic but clean (intrinsic) materials such as the optimally doped high-T_c layered cuprate superconductors. The calculated normal-state C-axis resistivity \rho_c(T) then follows the metal-like temperature dependence of the ab-plane resistivity \rho_{ab}(T) at high temperatures. At low enough temperatures, however, \rho_c(T) exhibits a non-metal like upturn even as \rho_{ab}(T) remains metallic. Moreover, in the metallic regime, \rho_c(T) is not limited by the maximum metallic resistivity of Mott-Ioffe-Regel. This correlation between the intrinsic \rho_c(T) and \rho_{ab}(T) is observed in the normal state of the high-T_c stoichiometric cuprates.",9704242v1 1997-09-24,Radiation Induced Damage in GaAs Particle Detectors,"The motivation for investigating the use of GaAs as a material for detecting particles in experiments for High Energy Physics (HEP) arose from its perceived resistance to radiation damage. This is a vital requirement for detector materials that are to be used in experiments at future accelerators where the radiation environments would exclude all but the most radiation resistant of detector types.",9709034v1 2017-07-05,Effects of Temperature and Near Ultraviolet Light on Current-Voltage Characteristics of Colemanite,"We investigate current-voltage (I-V) characteristics of the ferroelectric material colemanite at room temperature, at a high temperature, and also under the influence of near ultraviolet light. We demonstrate that all three I-V plots exhibit hysteresis effects, and these new results shed new light on the resistance of colemanite. These novel properties are explained on the basis of its microstructure indicating potential applications in devices with negative resistance as well as in photovoltaic devices.",1707.01194v1 2023-08-23,Verification of Wiedemann-Franz law in silver with moderate residual resistivity ratio,"Electrical and thermal transport were studied in a vacuum-annealed polycrystalline silver wire with residual resistivity ratio 200-400, in the temperature range 0.1-1.2K and in magnetic fields up to 5T. Both at zero field and at 5T the wire exhibits the Wiedemann-Franz law with the fundamental Lorenz number, contrary to an earlier report [Gloos, K. et al, Cryogenics 30, 14 (1990)]. Our result demonstrates that silver is an excellent material for thermal links in ultra-low-temperature experiments operating at high magnetic fields.",2308.12349v1 2016-02-02,Coexistence of magneto-resistance and -capacitance tunability in Sm2Ga2Fe2O9,"We propose that charge gradient resulting in the coexisting magneto-resistance and-capacitance tunability in material systems. We have experimentally observed coexisting of tunable magneto-resistance and -capacitance in Sm2Ga2Fe2O9. Our model fits well with the experimental result.",1602.01136v1 2013-03-06,Nonlinear Surface Resistance of YBa2Cu3O7-x Superconducting Thin Films on MgO Substrates in Dielectric Resonator at Ultra High Frequencies,"The nonlinear surface resistance Rs of the YBa2Cu3O7-x superconducting thin films on the MgO substrates was researched in the Hakki-Coleman dielectric resonator at the microwave signal powers from -18 dBm to +30 dBm at the ultra high frequency of 25 GHz in the range of temperatures from 12 K to 85 K. The dependences of the surface resistance on the temperature RS(T) in the YBa2Cu3O7-x superconducting thin films at the microwaves were measured. The dependence of the surface resistance on the microwave power RS(P) in the YBa2Cu3O7-x superconducting thin films at the microwaves were found at the two temperatures T = 25 K and T = 50 K. The full expression for the estimation of the measurements accuracy of the surface resistance RS was derived, and the measurements accuracy was set at 1 %. The physical mechanisms, which can be used to explain the experimental results, were discussed. It is shown that the surface resistance Rs can nonlinearly increase as a result of the transition by the sub-surface layer of the HTS thin film in a mixed state with the Abricosov and Josephson magnetic vortices generation at an increase of the microwave signal power P above the magnitude of 8 dBm. It is assumed that some additional energy losses have place, because of the microwave power dissipation on the normal metal cores of the magnetic vortices.",1303.1276v2 2019-12-13,Picosecond Multilevel Resistive Switching in Tantalum Oxide Thin Films,"The increasing demand for high-density data storage leads to an increasing interest in novel memory concepts with high scalability and the opportunity of storing multiple bits in one cell. A promising candidate is the redox-based resistive switch repositing the information in form of different resistance states. For reliable programming, the underlying physical parameters need to be understood. We reveal that the programmable resistance states are linked to internal series resistances and the fundamental nonlinear switching kinetics. The switching kinetics of Ta$_{2}$O$_{5}$-based cells was investigated in a wide range over 15 orders of magnitude from 250 ps to 10$^{5}$ s. We found strong evidence for a switching speed of 10 ps which is consistent with analog electronic circuit simulations. On all time scales, multi-bit data storage capabilities were demonstrated. The elucidated link between fundamental material properties and multi-bit data storage paves the way for designing resistive switches for memory and neuromorphic applications.",2002.00700v1 2014-03-05,Strong Oxidation Resistance of Atomically Thin Boron Nitride Nanosheets,"Investigation on oxidation resistance of two-dimensional (2D) materials is critical for many of their applications, because 2D materials could have higher oxidation kinetics than their bulk counterparts due to predominant surface atoms and structural distortions. In this study, the oxidation behavior of high-quality boron nitride (BN) nanosheets of 1-4 layer thick has been examined by heating in air. Atomic force microscopy and Raman spectroscopy analyses reveal that monolayer BN nanosheets can sustain up to 850 {\deg}C and the starting temperature of oxygen doping/oxidation of BN nanosheets only slightly increases with the increase of nanosheet layer and depends on heating conditions. Elongated etch lines are found on the oxidized monolayer BN nanosheets, suggesting that the BN nanosheets are first cut along the chemisorbed oxygen chains and then the oxidative etching grows perpendicularly to these cut lines. The stronger oxidation resistance of BN nanosheets suggests that they are more preferable for high-temperature applications than graphene.",1403.1002v1 2016-08-30,Design and Demonstration of Ultra Wide Bandgap AlGaN Tunnel Junctions,"Ultra violet light emitting diodes (UV LEDs) face critical limitations in both the injection efficiency and light extraction efficiency due to the resistive and absorbing p-type contact layers. In this work, we investigate the design and application of polarization engineered tunnel junctions for ultra-wide bandgap AlGaN (Al mole fraction higher than 50%) materials towards highly efficient UV LEDs. We demonstrate that polarization-induced 3D charge is beneficial in reducing tunneling barriers especially for high composition AlGaN tunnel junctions. The design of graded tunnel junction structures could lead to low tunneling resistance below 10-3 Ohm cm2 and low voltage consumption below 1 V (at 1 kA/cm2) for high composition AlGaN tunnel junctions. Experimental demonstration of 292 nm emission was achieved through non-equilibrium hole injection into wide bandgap materials with bandgap energy larger than 4.7 eV, and detailed modeling of tunnel junctions shows that they can be engineered to have low resistance, and can enable efficient emitters in the UV-C wavelength range.",1608.08653v1 2010-02-10,"Strain, magnetic anisotropy, and anisotropic magnetoresistance in (Ga,Mn)As on high-index substrates: application to (113)A-oriented layers","Based on a detailed theoretical examination of the lattice distortion in high-index epilayers in terms of continuum mechanics, expressions are deduced that allow the calculation and experimental determination of the strain tensor for (hhl)-oriented (Ga,Mn)As layers. Analytical expressions are derived for the strain-dependent free-energy density and for the resistivity tensor for monoclinic and orthorhombic crystal symmetry, phenomenologically describing the magnetic anisotropy (MA) and anisotropic magnetoresistance (AMR) by appropriate anisotropy and resistivity parameters, respectively. Applying the results to (113)A orientation with monoclinic crystal symmetry, the expressions are used to determine the strain tensor and the shear angle of a series of (113)A-oriented (Ga,Mn)As layers by high-resolution x-ray diffraction and to probe the MA and AMR at 4.2 K by means of angle-dependent magnetotransport. Whereas the transverse resistivity parameters are nearly unaffected by the magnetic field, the parameters describing the longitudinal resistivity are strongly field dependent.",1002.2179v2 2011-08-08,Beam screen issues,"In the High Energy LHC (HE-LHC), a beam energy of about 16.5 TeV is currently contemplated. The beam screen issues linked to the use of 20 T dipole magnets instead of 8.33 T are discussed, with a particular emphasis on two mechanisms, the magneto-resistance and the anomalous skin effect, assuming the nominal machine and beam parameters. The magneto-resistance effect always leads to an increase of the material resistivity (as the mean free path in the presence of a transverse magnetic field becomes smaller). As concerns the anomalous skin effect, the anomalous increase of surface resistance of metals at low temperatures and high frequencies is attributed to the long mean free path of the conduction electrons: when the skin depth becomes much smaller than the mean free path, only a fraction of the conduction electrons moving almost parallel to the metal surface is effective in carrying the current and the classical theory breaks down.",1108.1643v1 2012-04-15,A Structural Phase Transition in Ca3Co4O9 Associated with Enhanced High Temperature Thermoelectric Properties,"Temperature dependent electrical resistivity, crystal structure and heat capacity measurements reveal a resistivity drop and metal to semiconductor transition corresponding to first order structural phase transition near 400 K in Ca3Co4O9. The lattice parameter c varies smoothly with increasing temperature, while anomalies in the a, b1 and b2 lattice parameters occur at ~ 400 K. Both Ca2CoO3 and CoO2 layers become distorted above ~ 400 K associated with the metal to semiconductor transport behavior change. Resistivity and heat capacity measurements as a function of temperature under magnetic field indicates low spin contribution to this transition. Reduced resistivity associated with this first order phase transition from metallic to semiconducting behavior enhances the thermoelectric properties at high temperatures and points to the metal to semiconductor transition as a mechanism for improved ZT in high temperature thermoelectric oxides.",1204.3231v1 2015-10-07,Fabrication and Characterisation of Oil-Free Large High Pressure Laminate Resistive Plate Chamber,"A large (240 cm $\times$ 120 cm $\times$ 0.2 cm) oil-free High Pressure Laminate (HPL), commonly referred as ""bakelite"", Resistive Plate Chamber (RPC) has been developed at VECC-Kolkata using locally available P-302 OLTC grade HPL. The chamber has been operated in streamer mode using Argon, Freon(R134a) and Iso-butane in a ratio of 34:57:9 by volume. The electrodes and glue samples have been characterised by measuring their electrical parameters like bulk resistivity and surface resistivity. The performance of the chamber has been studied by measuring the efficiency, its uniformity and stability in detection of cosmic muons. Timing measurement has been performed at a central location of the chamber. The chamber showed an efficiency $>$95$\%$ and time resolution ($\sigma$), at the point of measurement, $\sim$0.83 ns at 9000V. Details of the material characterisation, fabrication procedure and performance studies have been discussed.",1510.02028v4 2016-11-22,CSAR 62 as negative-tone resist for high-contrast e-beam lithography at temperatures between 4 K and room temperature,"The temperature dependence of the electron-beam sensitive resist CSAR 62 is investigated in its negative-tone regime. The writing temperatures span a wide range from 4 K to room temperature with the focus on the liquid helium temperature regime. The importance of low temperature studies is motivated by the application of CSAR 62 for deterministic nanophotonic device processing by means of in-situ electron-beam lithography. At low temperature, CSAR 62 exhibits a high contrast of 10.5 and a resolution of 49 nm. The etch stability is almost temperature independent and it is found that CSAR 62 does not suffer from peeling which limits the low temperature application of the standard electron-beam resist PMMA. As such, CSAR 62 is a very promising negative-tone resist for in-situ electron-beam lithography of high quality nanostructures at low temperature.",1611.07266v1 2017-07-24,Advancement in the understanding of the field and frequency dependent microwave surface resistance of niobium,"The radio-frequency surface resistance of niobium resonators is incredibly reduced when nitrogen impurities are dissolved as interstitial in the material, conferring ultra-high Q-factors at medium values of accelerating field. This effect has been observed in both high and low temperature nitrogen treatments. As a matter of fact, the peculiar anti Q-slope observed in nitrogen doped cavities, i.e. the decreasing of the Q-factor with the increasing of the radio-frequency field, come from the decreasing of the BCS surface resistance component as a function of the field. Such peculiar behavior has been considered consequence of the interstitial nitrogen present in the niobium lattice after the doping treatment. The study here presented show the field dependence of the BCS surface resistance of cavities with different resonant frequencies, such as: 650 MHz, 1.3 GHz, 2.6 GHz and 3.9 GHz, and processed with different state-of-the-art surface treatments. These findings show for the first time that the anti Q-slope might be seen at high frequency even for clean Niobium cavities, revealing useful suggestion on the physics underneath the anti Q-slope effect.",1707.07582v1 2022-09-29,"Magnetic properties, electrical resistivity, and hardness of high-entropy alloys FeCoNiPd and FeCoNiPt","We report the magnetic properties, electrical resistivity, and Vickers microhardness of as-cast and annealed high-entropy alloys (HEAs) FeCoNiPd and FeCoNiPt with the face-centered cubic structure. The heat treatment at 800 $^{\circ}$C does not largely affect the physical properties in each HEA. The values of the Curie temperature and the saturation moment at 50 K are 955 K and 1.458 $\mu_\mathrm{B}$/f.u. for the annealed FeCoNiPd, and 851 K and 1.456 $\mu_\mathrm{B}$/f.u. for the annealed FeCoNiPt, respectively. Each HEA is a soft ferromagnet and shows metallic resistivity. The electronic structure calculations of both HEAs support the ferromagnetic ground states. The comparisons between experimental and theoretical values are made for the Curie temperature, the saturation moment, and the residual resistivity. The Vickers microhardness of annealed FeCoNiPd and FeCoNiPt are both 188 HV. The hardness vs. valence electron count (VEC) per atom plot of these HEAs does not largely deviate from an expected universal relation forming a broad peak at VEC$\sim$6.8. This study would give some hints on designing a soft ferromagnetic HEA with high hardness.",2209.14506v1 2018-11-29,Logarithmic Upturn in Low-Temperature Electronic Transport as a Signature of d-Wave Order in Cuprate Superconductors,"In cuprate superconductors, high magnetic fields have been used extensively to suppress superconductivity and expose the underlying normal state. Early measurements revealed insulating-like behavior in underdoped material versus temperature $T$, in which resistivity increases on cooling with a puzzling $\log(1/T)$ form. We instead use microwave measurements of flux-flow resistivity in YBa$_2$Cu$_3$O$_{6+y}$ and Tl$_2$Ba$_2$CuO$_{6+\delta}$ to study charge transport deep inside the superconducting phase, in the low temperature and low field regime. Here, the transition from metallic low-temperature resistivity ($d\rho/dT>0$) to a $\log(1/T)$ upturn persists throughout the superconducting doping range, including a regime at high carrier dopings in which the field-revealed normal-state resistivity is Fermi-liquid-like. The $\log(1/T)$ form is thus likely a signature of $d$-wave superconducting order, and the field-revealed normal state's $\log(1/T)$ resistivity may indicate the free-flux-flow regime of a phase-disordered $d$-wave superconductor.",1811.12348v1 2019-05-31,Pressure-Induced Structural Phase Transition and a Special Amorphization Phase of Two-Dimensional Ferromagnetic Semiconductor Cr2Ge2Te6,"Layered transition-metal trichalcogenides have become one of the research frontiers as two-dimensional magnets and candidate materials used for phase-change memory devices. Herein we report the high-pressure synchrotron X-ray diffraction and resistivity measurements on Cr2Ge2Te6 (CGT) single crystal by using diamond anvil cell techniques, which reveal a mixture of crystalline-to-crystalline and crystalline-to-amorphous transitions taking place concurrently at 18.3-29.2 GPa. The polymorphic transition could be interpreted by atomic layer reconstruction and the amorphization could be understood in connection with randomly flipping atoms into van der Waals gaps. The amorphous (AM) phase is quenchable to ambient conditions. The electrical resistance of CGT shows a bouncing point at ~ 18 GPa, consistent with the polymorphism phase transition. Interestingly, the high-pressure AM phase exhibits metallic resistance with the magnitude comparable to that of high-pressure crystalline phases, whereas the resistance of the AM phase at ambient pressure fails to exceed that of the crystalline phase, indicating that the AM phase of CGT appeared under high pressure is quite unique and similar behavior has never been observed in other phase-change materials. The results definitely would have significant implications for the design of new functional materials.",1905.13603v1 2018-08-23,Evidence for superconductivity above 260 K in lanthanum superhydride at megabar pressures,"Recent predictions and experimental observations of high Tc superconductivity in hydrogen-rich materials at very high pressures are driving the search for superconductivity in the vicinity of room temperature. We have developed a novel preparation technique that is optimally suited for megabar pressure syntheses of superhydrides using pulsed laser heating while maintaining the integrity of sample-probe contacts for electrical transport measurements to 200 GPa. We detail the synthesis and characterization, including four-probe electrical transport measurements, of lanthanum superhydride samples that display a significant drop in resistivity on cooling beginning around 260 K and pressures of 190 GPa. Additional measurements on two additional samples synthesized the same way show resistance drops beginning as high as 280 K at these pressures. The loss of resistance at these high temperatures is not observed in control experiments on pure La as well as in partially transformed samples at these pressures, and x-ray diffraction as a function of temperature on the superhydride reveal no structural changes on cooling. We infer that the resistance drop is a signature of the predicted room-temperature superconductivity in LaH10, in good agreement with density functional structure search and BCS theory calculations.",1808.07695v3 2021-02-04,Enhancing plasticity in high-entropy refractory ceramics via tailoring valence electron concentration,"Bottom-up design of high-entropy ceramics is a promising approach for realizing materials with unique combination of high hardness and fracture-resistance at elevated temperature. This work offers a simple yet fundamental design criterion - valence electron concentration (VEC) > ~9.5 e-/f.u. to populate bonding metallic states at the Fermi level - for selecting elemental compositions that may form rocksalt-structure (B1) high-entropy ceramics with enhanced plasticity (reduced brittleness). Single-phase B1 (HfTaTiWZr)C and (MoNbTaVW)C, chosen as representative systems due to their specific VEC values, are here synthesized and tested. Nanoindentation arrays at various loads and depths statistically show that (HfTaTiWZr)C (VEC=8.6 e-/f.u.) is hard but brittle, whilst (MoNbTaVW)C (VEC=9.4 e-/f.u.) is hard and considerably more resistant to fracture than (HfTaTiWZr)C. Ab initio molecular dynamics simulations and electronic-structure analysis reveal that the improved fracture-resistance of (MoNbTaVW)C subject to tensile and shear deformation may originate from the intrinsic material's ability to undergo local lattice transformations beyond tensile yield points, as well as from relatively facile activation of lattice slip. Additional simulations, carried out to follow the evolution in mechanical properties as a function of temperature, suggest that (MoNbTaVW)C may retain good resistance to fracture up to ~900-1200K, whereas (HfTaTiWZr)C is predicted to remain brittle at all investigated temperatures.",2102.02455v2 2020-09-08,High-Pressure Torsion Deformation Induced Phase Transformations and Formations: New Material Combinations and Advanced Properties,"Heavy plastic shear deformation at relatively low homologous temperatures is called high-pressure torsion (HPT) deformation, which is one method of severe plastic deformation (SPD). The aim of the paper is to give an overview of a new processing approach which permits the generation of innovative metastable materials and novel nanocomposites by HPT deformation. Starting materials can be either coarse-grained multi-phase alloys, a mixture of different elemental powders or any other combination of multiphase solid starting materials. After HPT processing, the achievable microstructures are similar to the ones generated by mechanical alloying. Nevertheless, one advantage of the HPT process is that bulk samples of the different types of metastable materials and nanocomposites are obtained directly during HPT deformation. It will be shown that different material combinations can be selected and materials with tailored properties, or in other words, materials designed for specific applications and the thus required properties, can be synthesized. Areas of application for these new materials range from hydrogen storage to materials resistant to harsh radiation environments.",2009.03531v1 2023-12-08,Low Resistance Ohmic Contact to P-type Monolayer WSe2,"Advanced microelectronics in the future may require semiconducting channel materials beyond silicon. Two-dimensional (2D) semiconductors, characterized by their atomically thin thickness, hold immense promise for high-performance electronic devices at the nanometer scale with lower heat dissipation. One challenge for achieving high-performance 2D semiconductor field effect transistors (FET), especially for p-type materials, is the high electrical contact resistance present at the metal-semiconductor interface. In conventional bulk semiconductors, low resistance ohmic contact is realized through heavy substitutional doping with acceptor or donor impurities at the contact region. The strategy of substitutional doping, however, does not work for p-type 2D semiconductors such as monolayer tungsten diselenide (WSe$_2$).In this study, we developed highly efficient charge-transfer doping with WSe$_2$/$\alpha$-RuCl$_3$ heterostructures to achieve low-resistance ohmic contact for p-type WSe$_2$ transistors. We show that a hole doping as high as 3$\times$10$^{13}$ cm$^{-2}$ can be achieved in the WSe$_2/\alpha$-RuCl$_3$ heterostructure due to its type-III band alignment. It results in an Ohmic contact with resistance lower than 4 k Ohm $\mu$m at the p-type monolayer WSe$_2$/metal junction. at room temperature. Using this low-resistance contact, we demonstrate high-performance p-type WSe$_2$ transistors with a saturation current of 35 $\mu$A$\cdot$ $\mu$m$^{-1}$ and an I$_{ON}$/I$_{OFF}$ ratio exceeding 10$^9$ It could enable future microelectronic devices based on 2D semiconductors and contribute to the extension of Moore's law.",2312.04849v1 2022-01-06,Model-based quantitative methods to predict irradiation-induced swelling in alloys,"Predicting volume swelling of structural materials in nuclear reactors under high-dose neutron irradiations based on existing low-dose experiments or irradiation data with high-dose-rate energetic particles has been a long-standing challenge for safety evaluation and rapidly screening irradiation-resistant materials in nuclear energy systems. Here, we build an Additional Defect Absorption Model that describes the irradiation-induced swelling effects produced by energetic electrons, heavy-ions, and neutrons by considering additional defect sinks inherent in the irradiation process. Based on this model, we establish quantitative methods to predict high-dose swelling from low-dose behavior and obtain the equivalent irradiation dose for different energetic particles when the dose rates differ by several orders of magnitude. Furthermore, we propose a universal parameter to characterize the swelling resistance of various alloys and predict their radiation tolerances under different radiation conditions. This work provides quantitative prediction methods for evaluating irradiation-induced swelling effects of structural materials, which is critical to the safety and material development for advanced nuclear reactors.",2201.04958v1 2022-10-28,An innovative materials design protocol for the development of novel refractory high-entropy alloys for extreme environments,"In the quest of new materials that can withstand severe irradiation and mechanical extremes for advanced applications (e.g. fission reactors, fusion devices, space applications, etc), design, prediction and control of advanced materials beyond current material designs become a paramount goal. Here, though a combined experimental and simulation methodology, the design of a new nanocrystalline refractory high entropy alloy (RHEA) system is established. Compositions of this alloy, assessed under extreme environments and in situ electron-microscopy, revealed both high mechanical strength and thermal stability, grain refinement under heavy ion irradiation and outstanding irradiation resistance to dual-beam irradiation and helium implantation, marked by remarkable resistance to defect generation, growth and coalescence. The experimental and modeling results, which demonstrated notable agreement, can be applied to design and rapidly assess other alloys subjected to extreme environmental conditions.",2210.16409v1 2023-02-07,Effect of ZrB$_2$ additions on the thermal stability of polycrystalline diamond,"This study investigates the effect of ZrB$_2$ additions on the microstructure, thermal stability, and thermo-mechanical wear behaviour of polycrystalline diamond. Following high-pressure high-temperature (HPHT) sintering, the ZrB$_2$-PCD material showed a full conversion of the binder phase to cobalt-boride (Co2B and Co$_{23}$B$_6$) phases. In-situ PXRD and TEM vacuum annealing experiments observed that the onset of bulk graphitisation occurred above $1000^{\circ}C$ for the ZrB$_2$-PCD material, compared to $850^{\circ}C$ for the STD-PCD material. The ZrB$_2$-PCD tools showed excellent thermo-mechanical wear behaviour, exhibiting increased durability and a steady wear scar progression during high-temperature dry-VTL testing. However, lowered abrasion wear resistance was observed for the ZrB2-PCD tools during low-temperature wet-VTL testing, probably due the reduced diamond contiguity in the ZrB2 additive sample. Further optimisation of the ZrB$_2$ additive phase content, mixing methodology, or sintering conditions could be explored to improve the abrasive wear resistance of this novel PCD material.",2302.03464v1 2016-06-14,Origin of the metal-to-insulator crossover in cuprate superconductors,"Superconductivity in cuprates peaks in the doping regime between a metal at high p and an insulator at low p. Understanding how the material evolves from metal to insulator is a fundamental and open question. Early studies in high magnetic fields revealed that below some critical doping an insulator-like upturn appears in the resistivity of cuprates at low temperature, but its origin has remained a puzzle. Here we propose that this 'metal-to-insulator crossover' is due to a drop in carrier density n associated with the onset of the pseudogap phase at a critical doping p*. We use high-field resistivity measurements on LSCO to show that the upturns are quantitatively consistent with a drop from n=1+p above p* to n=p below p*, in agreement with high-field Hall data in YBCO. We demonstrate how previously reported upturns in the resistivity of LSCO, YBCO and Nd-LSCO are explained by the same universal mechanism: a drop in carrier density by 1.0 hole per Cu atom.",1606.04491v1 2020-05-30,Linearity and rate capability measurements of RPC with semi-insulating crystalline electrodes operating in avalanche mode,"The intrinsic rate capability and the ageing properties of the Resistive Plate Chambers are closely related to the electrodes material and to the front-end electronics threshold. The development of a low noise pre-amplifier led us to improve the intrinsic rate capability of High Pressure Laminate (bakelite) up to $\sim10\;kHz/cm^2$, nevertheless the effective rate is significantly limited by electrodes ageing. To further improve the effective rate capability new materials are investigated. A Resistive Plate Chamber with crystalline semi-insulating Gallium Arsenide electrodes has been characterized with high energy electrons beam at the Beam Test Facility (BFT), (INFN National Laboratory of Frascati, Italy). The response of the Resistive Plate Chamber to multiple bunched electrons was measured operating the detector in avalanche mode. The intrinsic rate capability has been also measured operating the detector in a uniform high energy gamma radiation field at the GIF++ facility (EHN1 of SPS, CERN).",2006.00306v1 2016-06-17,Manganite-based three level memristive devices with self-healing capability,"We report on non-volatile memory devices based on multifunctional manganites. The electric field induced resistive switching of Ti/$La_{1/3}$$Ca_{2/3}$Mn$O_3$/n-Si devices is explored using different measurement protocols. We show that using current as the electrical stimulus (instead of standard voltage-controlled protocols) improves the electrical performance of our devices and unveils an intermediate resistance state. We observe three discrete resistance levels (low, intermediate and high), which can be set either by the application of current-voltage ramps or by means of single pulses. These states exhibit retention and endurance capabilities exceeding $10^4$ s and 70 cycles, respectively. We rationalize our experimental observations by proposing a mixed scenario were a metallic filament and a Si$O_x$ layer coexist, accounting for the observed resistive switching. Overall electrode area dependence and temperature dependent resistance measurements support our scenario. After device failure takes place, the system can be turned functional again by heating up to low temperature (120 C), a feature that could be exploited for the design of memristive devices with self-healing functionality. These results give insight into the existence of multiple resistive switching mechanisms in manganite-based memristive systems and provide strategies for controlling them.",1606.05401v1 2019-07-25,Extraction of the short-range defect potential parameters from available experimental data on the graphene resistance,"We consider a problem of obtaining information about the scattering potentials of the monolayer graphene sample using available experimental data on its resistance. We have in mind a development of the study describing super-high mobility electrons in suspended samples without chemical doping. As far as practical absence of the doping impurities in this case makes the Coulomb scattering negligible, we consider models of the short-range scattering potentials. The model of short-range potential is assumed to be supported by the close vicinity of the ring or the circumference of a circle. The diameter of circles is supposed to be of the order of the crystal lattice spacing. The empty core of the model potential guarantees the suppression of nonphysical shortwave modes. Two models are investigated: the delta function on the circumference of a circle (delta shell) and the annual well. An advantage of the former is simplicity, while a virtue of the latter is regularity. We consider scattering of electrons by these potentials and obtain exact explicit formulae for the scattering data. We here discuss application of these formulae for calculation of observables. Namely, we analyze the contribution of this scattering into the graphene resistance and plot the resistivity as a function of the Fermi energy according to our theoretical formulae. The obtained results are consistent with experiment, where the resistance was measured as a function of the Fermi momentum on the suspended annealed graphene. This fact gives a possibility to find parameters of the modeled potential on the base of the available experimental data on resistance of the suspended graphene sample with the gate voltage controlled Fermi level position. It is clear to be very important for applications.",1907.10894v1 2021-08-23,Polarization and resistive switching in epitaxial 2 nm Hf$_{0.5}$Zr$_{0.5}$O$_2$ tunnel junctions,"In the quest for reliable and power-efficient memristive devices, ferroelectric tunnel junctions are being investigated as potential candidates. CMOS-compatible ferroelectric hafnium oxides are at the forefront. However, in epitaxial tunnel devices with thicknesses around ${\approx}$ 4 - 6 nm, the relatively high tunnel energy barrier produces a large resistance that challenges their implementation. Here, we show that ferroelectric and electroresistive switching can be observed in ultrathin 2 nm epitaxial Hf$_{0.5}$Zr$_{0.5}$O$_2$ (HZO) tunnel junctions in large area capacitors (${\approx} 300{\mu}m^2$). We observe that the resistance area product is reduced to about 160 ${\Omega}{\cdot}$cm$^2$ and 65 ${\Omega}{\cdot}$cm$^2$ for OFF and ON resistance states, respectively. These values are two orders of magnitude smaller than those obtained in equivalent 5 nm HZO tunnel devices while preserving a similar OFF/ON resistance ratio (210 ${\%}$). The devices show memristive and spike-timing-dependent plasticity (STDP) behavior and good retention. Electroresistance and ferroelectric loops closely coincide, signaling ferroelectric switching as a driving mechanism for resistance change.",2108.10373v1 2002-08-18,Synthesis and physical properties of LiBC intermetallics,"Polycrystalline samples of LiBC compounds, which were predicted as possible candidate for high-Tc superconductivity, have been synthesised by a flux method and investigated by means of electrical resistivity and magnetic susceptibility. Scanning electron microscopy and X-ray diffraction patterns showed a plate-like morphology and a single-phase nature of LiBC samples for starting composition of Li1.25BC (flux composition). The lattice constants a, c display a systematic variation with x and has maximum volume of the hexagonal unit cell at x = 1.25. Electrical resistivity measurements revealed an extrinsic semi-conducting behaviour of the single-phase LiBC with an activation energy of 18 meV and a maximum specific resistivity of 2.5 Wcm at 300 K. In contrast to the theoretical prediction of high Tc, no superconducting features were detected down to 2 K both, by measurements of electrical resistivity and magnetic susceptibility.",0208346v2 2008-10-22,Quantum resistance metrology in graphene,"We have performed a metrological characterization of the quantum Hall resistance in a 1 $\mu$m wide graphene Hall-bar. The longitudinal resistivity in the center of the $\nu=\pm 2$ quantum Hall plateaus vanishes within the measurement noise of 20 m$\Omega$ upto 2 $\mu$A. Our results show that the quantization of these plateaus is within the experimental uncertainty (15 ppm for 1.5$ \mu$A current) equal to that in conventional semiconductors. The principal limitation of the present experiments are the relatively high contact resistances in the quantum Hall regime, leading to a significantly increased noise across the voltage contacts and a heating of the sample when a high current is applied.",0810.4064v1 2011-02-14,"Coexistence of superconductivity and antiferromagnetism in single crystals $A_{0.8}Fe_{2-y}Se_2$ (A= K, Rb, Cs, Tl/K and Tl/Rb): evidence from magnetization and resistivity","We measure the resistivity and magnetic susceptibility in the temperature range from 5 K to 600 K for the single crystals $A$Fe$_{2-y}$Se$_2$ ($A$ = K$_{0.8}$, Rb$_{0.8}$, Cs$_{0.8}$, Tl$_{0.5}$K$_{0.3}$ and Tl$_{0.4}$Rb$_{0.4}$). A sharp superconducting transition is observed in low temperature resistivity and susceptibility, and susceptibility shows 100% Meissner volume fraction for all crystals, while an antiferromagnetic transition is observed in susceptibility at Neel temperature ($T_N$) as high as 500 K to 540 K depending on A. It indicates the coexistence of superconductivity and antiferromagnetism. A sharp increase in resistivity arises from the structural transition due to Fe vacancy ordering at the temperature slightly higher than $T_{\rm N}$. Occurrence of superconductivity in an antiferromagnetic ordered state with so high $T_{\rm N}$ may suggest new physics in this type of unconventional superconductors.",1102.2783v1 2012-08-15,Two-dimensional electron-gas-like charge transport at magnetic Heusler alloy-SrTiO$_3$ interface,"We report remarkably low residual resistivity, giant residual resistivity ratio, free-electron-like Hall resistivity and high mobility ($\approx$ 10$^4$ cm$^2$V$^{-1}$s$^{-1}$) charge transport in epitaxial films of Co$_2$MnSi and Co$_2$FeSi grown on (001) SrTiO$_3$. This unusual behavior is not observed in films deposited on other cubic oxide substrates of comparable lattice parameters. The scaling of the resistivity with thickness of the films allow extraction of interface conductance, which can be attributed to a layer of oxygen vacancies confined within 1.9 nm of the interface as revealed by atomically resolved electron microscopy and spectroscopy. The high mobility transport observed here at the interface of a fully spin polarized metal is potentially important for spintronics applications.",1208.3099v2 2014-10-29,Large time-dependent coercivity and resistivity modification under sustained voltage application in a Pt/Co/AlOx/Pt junction,"The coercivity and resistivity of a Pt/Co/AlOx/Pt junction are measured under sustained voltage application. High bias voltages of either polarity are determined to cause a strongly enhanced, reversible coercivity modification compared to low voltages. Time-resolved measurements show a logarithmic development of the coercive field in this regime, which continues over a period as long as thirty minutes. Furthermore, the resistance of the dielectric barrier is found to change strongly and reversibly on the same time scale, suggesting an electrochemical process is taking place within the dielectric. It is argued that the migration of oxygen vacancies at the magnet/oxide interface could explain both the resistance variation and the enhanced electric field effect at high voltages. A thermal fluctuation aftereffect model is applied to account for the observed logarithmic dependence.",1410.8018v1 2017-06-29,Effect of Anodizing Parameters on Corrosion Resistance of Coated Purified Magnesium,"Magnesium and its alloys are being considered for biodegradable biomaterials. However, high and uncontrollable corrosion rates have limited the use of magnesium and its alloys in biological environments. In this research, high purified magnesium (HP-Mg) was coated with stearic acid in order to improve the corrosion resistance of magnesium. Anodization and immersion in stearic acid were used to form a hydrophobic layer on magnesium substrate. Different DC voltages, times, electrolytes, and temperatures were tested. Electrochemical impedance spectroscopy and potentiodynamic polarization were used to measure the corrosion rates of the coated HP-Mg. The results showed that optimum corrosion resistance occurred for specimens anodized at +4 volts for 4 minutes at 70{\deg}C in borate benzoate. The corrosion resistance was temporarily enhanced by 1000x.",1706.09547v1 2017-12-08,Selective etching of PDMS: etching as a negative tone resist,"In this work authors present for the first time how to apply the additive-free, cured PDMS as a negative tone resist material, demonstrate the creation of PDMS microstructures and test the solvent resistivity of the created microstructures. The PDMS layers were 45 um and 100 um thick, the irradiations were done with a focused proton microbeam with various fluences. After irradiation, the samples were etched with sulfuric acid that removed the unirradiated PDMS completely but left those structures intact that received high enough fluences. The etching rate of the unirradiated PDMS was also determined. Those structures that received at least 7.5*10^15 ion*cm-2 fluence did not show any signs of degradation even after 19 hours of etching. As a demonstration, 45 um and 100 um tall, high aspect ratio, good quality, undistorted microstructures were created with smooth and vertical sidewalls. The created microstructures were immersed into numerous solvents and some acids to test their compatibility. It was found that the unirradiated PDMS cannot, while the irradiated PDMS microstructures can resist to chloroform, n-hexane, toluene and sulfuric acid. Hydrogen fluoride etches both the unirradiated and the irradiated PDMS.",1712.03119v1 2018-06-28,Band-edge quasiparticles from electron phonon coupling and resistivity saturation,"We address the problem of resistivity saturation observed in materials such as the A-15 compounds. To do so, we calculate the resistivity for the Hubbard-Holstein model in infinite spatial dimensions to second order in on-site repulsion $U\leq D$ and to first order in (dimensionless) electron-phonon coupling strength $\lambda\leq0.5$, where $D$ is the half-bandwidth. We identify a unique mechanism to obtain two parallel quantum conducting channels: low-energy and band-edge high-energy quasi-particles. We identify the source of the hitherto unremarked high-energy quasi-particles as a positive slope in the frequency-dependence of the real part of the electron self-energy. In the presence of phonons, the self-energy grows linearly with the temperature at high-$T$, causing the resistivity to saturate. As $U$ is increased, the saturation temperature is pushed to higher values, offering a mechanism by which electron-correlations destroy saturation.",1806.11227v2 2019-06-15,Unidirectional Synapse-Like Behavior of Zr/ZrO2-NT/Au Layered Structure,"Zirconia nanotubular layer with an outer tube diameter 25 nm was synthesized by potentiostatic anodization. The Zr/ZrO2-NT/Au memristive structure is fabricated using stencil mask and magnetron sputtering techniques. Current-voltage characteristics are measured in full cycles of resistive switching with varying parameters of the applied harmonic voltage. An equivalent circuit with unidirectional electrical conductivity for the studied structure is proposed. Estimates of the electrical resistance of memristors in high-and intermediate resistivity states are performed. The high synaptic plasticity of memristors based on the Zr/ZrO2-NT/Au structure is shown.",1906.06549v1 2019-06-25,Compositionally graded contact layers for MOCVD grown high Al-content AlGaN transistors,"In this letter, we design and demonstrate an improved MOCVD grown reverse Al-composition graded contact layer to achieve low resistance contact to MOCVD grown ultra-wide bandgap (UWBG) Al0.70Ga0.30N channel metal semiconductor field-effect transistors (MESFETs). Increasing the thickness of the reverse graded layer was found to improve contact layer resistance significantly, leading to contact resistance of 3.3x10^-5 Ohm.cm2. Devices with gate length, LG, of 0.6 microns and source-drain spacing, LSD, of 1.5 microns displayed a maximum current density, IDSMAX, of 635 mA/mm with an applied gate voltage, VGS, of +2 V. Breakdown measurements on transistors with gate to drain spacing, LGD, of 770 nm had breakdown voltage greater than 220 , corresponding to minimum breakdown field of 2.86 MV/cm. This work provides a framework for the design of low resistance contacts to MOCVD grown high Al-content AlxGa1-xN channel transistors.",1906.10270v2 2021-02-05,Formation of Ultra-High-Resistance Au/Ti/p-GaN Junctions and the Applications in AlGaN/GaN HEMTs,"We report a dramatic current reduction, or a resistance increase, by a few orders of magnitude of two common-anode Au/Ti/pGaN Schottky junctions annealed within a certain annealing condition window (600 - 700 oC, 1 - 4 min). Results from similar common-anode Schottky junctions made of Au/p-GaN, Al/Ti/p-GaN and Au/Ti/graphene/p-GaN junctions demonstrated that all the three layers (Au, Ti and p-GaN) are essential for the increased resistance. Raman characterization of the p-GaN showed a decrease of the Mg-N bonding, i.e., the deactivation of Mg, which is consistent with the Hall measurement results. Moreover, this high-resistance junction structure was employed in p-GaN gate AlGaN/GaN HEMTs. It was shown to be an effective gate technology that was capable to boost the gate breakdown voltage from 9.9 V to 13.8 V with a negligible effect on the threshold voltage or the sub-threshold slope.",2102.03418v1 2021-12-02,Homes' law in holographic superconductor with linear-$T$ resistivity,"Homes' law, $\rho_{s} = C \, \sigma_{DC} \, T_{c}$, is a universal relation of superconductors between the superfluid density $\rho_{s}$ at zero temperature, the critical temperature $T_{c}$ and the electric DC conductivity $\sigma_{DC}$ at $T_c$. Experimentally, Homes' law is observed in high $T_c$ superconductors with linear-$T$ resistivity in the normal phase, giving a material independent universal constant $C$. By using holographic models related to the Gubser-Rocha model, we investigate how Homes' law can be realized together with linear-$T$ resistivity in the presence of momentum relaxation. We find that strong momentum relaxation plays an important role to exhibit Homes' law with linear-$T$ resistivity.",2112.01153v2 2004-02-02,Universal charge transport of the Mn oxides in the high temperature limit,"We have found that various Mn oxides have the universal resistivity and thermopower in the high temperature limit. The resistivities and thermopowers of all the samples go toward constant values of 7$\pm$1 m$\Omega$cm and $-79\pm$3 $\mu$V/K, which are independent of carrier density and crystal structures. We propose that the electric conduction occurs in a highly localized way in the high temperature limit, where the exchange of entropy and charge occurs in the neighboring Mn$^{3+}$ and Mn$^{4+}$ ions.",0402032v1 2009-05-19,Boosting electronic transport in carbon nanotubes by isotopic disorder,"The current/voltage curve of metallic carbon nanotubes (CNTs) displays at high bias a sudden increase of the resistivity due to the scattering of electrons with phonons having an anomalously-high population (hot phonons). Here, we show that it is possible to improve the electrical performances of metallic CNTs by C13 isotope enrichment. In fact, isotopic disorder creates additional channels for the hot-phonon deexcitation, reduces their population and, thus, the nanotube high-bias differential-resistance. This is an extraordinary case where disorder improves the electronic transport.",0905.3034v1 2011-04-05,Effect of uniaxial stress on low-frequency dispersion of dielectric constant in high-resistivity GaSe crystals,"Low-frequency dielectric spectra of high-resistivity GaSe layered crystals have been studied on the samples clamped between two insulating parallel plates at frequencies up to 100 kHz. The measurements have been carried out at different uniaxial stresses up to $2.4\times10^5$ Pa applied along the c-axis normal to crystal layer's plane. It is revealed that the dielectric spectra of high-resistivity GaSe layered crystals with insulating plates obey a universal power law ${\sim}\omega^{n-1}$, where ${\omega}$ is the angular frequency and $n\approx 0.8$, earlier observed on high-resistivity GaSe crystals with indium-soldered contacts. The same type of spectra on the crystals with different types of contacts (insulating and ohmic) confirms the bulk character of the observed polarization caused by hopping charge carriers. It is shown that the frequency-dependent dielectric constant increases linearly with the uniaxial stress characterized by the coefficient ${\Delta}{\epsilon}/({\epsilon}{\Delta}{p})=8{\times}10^{-7}$ Pa$^{-1}$. A slight increase of power $1-n$ with the stress is observed, that leads to a stronger dielectric dispersion. The strong stress dependence of the low-frequency dielectric constant in high-resistivity GaSe crystals may be referred to the presence of the formations of elementary dipoles, rotations of which correspond to hops of localized charge carriers.",1104.0801v1 2017-12-08,Selective etching of PDMS: etching as positive resist,"Although, poly(dimethylsiloxane) (PDMS) is a widely used material in numerous applications, such as micro- or nanofabrication, the method of its selective etching has not been known up to now. In this work authors present two methods of etching the pure, additive-free and cured PDMS as a positive resist material. To achieve the chemical modification of the polymer necessary for selective etching, energetic ions were used. We created 7 um and 45 um thick PDMS layers and patterned them by a focused proton microbeam with various, relatively large fluences. In this paper authors demonstrate that 30 wt% Potassium Hydroxide (KOH) or 30 wt% sodium hydroxide (NaOH) at 70 oC temperature etch proton irradiated PDMS selectively, and remove the chemically sufficiently modified areas. In case of KOH development, the maximum etching rate was approximately 3.5 um/minute and it occurs at about 7.5*10^15 ion*cm-2. In case of NaOH etching the maximum etching rate is slightly lower, 1.75 um/minute and can be found at the slightly higher fluence of 8.75*10^15 ion*cm-2. These results are of high importance since up to this time it has not been known how to develop the additive-free, cross-linked poly(dimethylsiloxane) in lithography as a positive tone resist material.",1712.03125v1 2021-04-14,Inverse design of glass structure with deep graph neural networks,"Directly manipulating the atomic structure to achieve a specific property is a long pursuit in the field of materials. However, hindered by the disordered, non-prototypical glass structure and the complex interplay between structure and property, such inverse design is dauntingly hard for glasses. Here, combining two cutting-edge techniques, graph neural networks and swap Monte Carlo, we develop a data-driven, property-oriented inverse design route that managed to improve the plastic resistance of Cu-Zr metallic glasses in a controllable way. Swap Monte Carlo, as ""sampler"", effectively explores the glass landscape, and graph neural networks, with high regression accuracy in predicting the plastic resistance, serves as ""decider"" to guide the search in configuration space. Via an unconventional strengthening mechanism, a geometrically ultra-stable yet energetically meta-stable state is unraveled, contrary to the common belief that the higher the energy, the lower the plastic resistance. This demonstrates a vast configuration space that can be easily overlooked by conventional atomistic simulations. The data-driven techniques, structural search methods and optimization algorithms consolidate to form a toolbox, paving a new way to the design of glassy materials.",2104.06632v3 2021-05-07,Integrating superconducting van der Waals materials on paper substrates,"Paper has the potential to dramatically reduce the cost of electronic components. In fact, paper is 10 000 times cheaper than crystalline silicon, motivating the research to integrate electronic materials on paper substrates. Among the different electronic materials, van der Waals materials are attracting the interest of the scientific community working on paper-based electronics because of the combination of high electrical performance and mechanical flexibility. Up to now, different methods have been developed to pattern conducting, semiconducting and insulating van der Waals materials on paper but the integration of superconductors remains elusive. Here, the deposition of NbSe2, an illustrative van der Waals superconductor, on standard copy paper is demonstrated. The deposited NbSe2 films on paper display superconducting properties (e.g. observation of Meissner effect and resistance drop to zero-resistance state when cooled down below its critical temperature) similar to those of bulk NbSe2.",2105.03487v1 2016-01-17,Resistivity plateau and extremely large magnetoresistance in NbAs2 and TaAs2,"In topological insulators (TIs), metallic surface conductance saturates the insulating bulk resistance with de- creasing temperature, resulting in resistivity plateau at low temperatures as a transport signature originating from metallic surface modes protected by time reversal symmetry (TRS). Such characteristic has been found in several materials including Bi2Te2Se, SmB6 etc. Recently, similar behavior has been observed in metallic com- pound LaSb, accompanying an extremely large magetoresistance (XMR). Shubnikov-de Hass (SdH) oscillation at low temperatures further confirms the metallic behavior of plateau region under magnetic fields. LaSb[1] has been proposed by the authors as a possible topological semimetal (TSM), while negative magnetoresistance is absent at this moment. Here, high quality single crystals of NbAs2/TaAs2 with inversion symmetry have been grown and the resistivity under magnetic field is systematically investigated. Both of them exhibit metallic behavior under zero magnetic field, and a metal-to-insulator transition occurs when a nonzero magnetic field is applied, resulting in XMR (1.0*105% for NbAs2 and 7.3*105% for TaAs2 at 2.5 K & 14 T). With tempera- ture decreased, a resistivity plateau emerges after the insulator-like regime and SdH oscillation has also been observed in NbAs2 and TaAs2.",1601.04239v1 2018-09-26,Changes in the near edge X-ray absorption fine structure of hybrid organic-inorganic resists upon exposure,"We report on the near edge X-ray absorption fine structure (NEXAFS) spectroscopy of hybrid organic-inorganic resists. These materials are nonchemically amplified systems based on Si, Zr, and Ti oxides, synthesized from organically modified precursors and transition metal alkoxides by a sol-gel route and designed for ultraviolet, extreme ultraviolet and electron beam lithography. The experiments were conducted using a scanning transmission X-ray microscope (STXM) which combines high spatial-resolution microscopy and NEXAFS spectroscopy. The absorption spectra were collected in the proximity of the carbon edge (~ 290 eV) before and after in situ exposure, enabling the measurement of a significant photo-induced degradation of the organic group (phenyl or methyl methacrylate, respectively), the degree of which depends on the configuration of the ligand. Photo-induced degradation was more efficient in the resist synthesized with pendant phenyl substituents than it was in the case of systems based on bridging phenyl groups. The degradation of the methyl methacrylate group was relatively efficient, with about half of the initial ligands dissociated upon exposure. Our data reveal that the such dissociation can produce different outcomes, depending on the structural configuration. While all the organic groups were expected to detach and desorb from the resist in their entirety, a sizeable amount of them remain and form undesired byproducts such as alkene chains. In the framework of the materials synthesis and engineering through specific building blocks, these results provide a deeper insight into the photochemistry of resists, in particular for extreme ultraviolet lithography.",1809.09916v1 2022-04-30,A simple strategy to measure the contact resistance between metals and doped organic films,"Charge injection from electrodes into doped organic films is a widespread technology used in the majority of state-of-the-art organic semiconductor devices. Although such interfaces are commonly considered to form Ohmic contacts via strong band bending, an experiment that directly measures the contact resistance has not yet been demonstrated. In this study, we use a simple metal/doped organic semiconductor/metal stack and study its voltage-dependent resistance. A transport layer thickness variation proves that the presented experiment gains direct access to the contact resistance of the device. We can quantify that for an operating current density of 10mA/cm2 the investigated material system exhibits a voltage drop over the metal/organic interface of about 200mV, which can be reduced by more than one order of magnitude when employing an additional injection layer. The presented experiment proposes a simple strategy to measure the contact resistance between any metal and doped organic film without applying numerical tools or elaborate techniques. Furthermore, the simplistic device architecture allows for very high, homogeneous, and tunable electric fields within the organic layer, which enables a clear investigation of the Poole-Frenkel effect.",2205.00261v1 2018-01-30,Novel circuit design for high-impedance and non-local electrical measurements of two-dimensional materials,"Two-dimensional materials offer a novel platform for the development of future quantum technologies. However, the electrical characterisation of topological insulating states, non-local resistance and bandgap tuning in atomically-thin materials, can be strongly affected by spurious signals arising from the measuring electronics. Common-mode voltages, dielectric leakage in the coaxial cables and the limited input impedance of alternate-current amplifiers can mask the true nature of such high-impedance states. Here, we present an optical isolator circuit which grants access to such states by electrically decoupling the current-injection from the voltage-sensing circuitry. We benchmark our apparatus against two state-of-the-art measurements: the non-local resistance of a graphene Hall bar and the transfer characteristic of a WS2 field-effect transistor. Our system allows the quick characterisation of novel insulating states in two-dimensional materials with potential applications in future quantum technologies.",1801.10135v1 2013-08-31,Origin of defects responsible for charge transport in resistive random access memory based on hafnia,"A promising candidate for universal memory, which would involve combining the most favourable properties of both high-speed dynamic random access memory (DRAM) and non-volatile flash memory, is resistive random access memory (ReRAM). ReRAM is based on switching back and forth from a high-resistance state (HRS) to a low-resistance state (LRS). ReRAM cells are small, allowing for the creation of memory on the scale of terabits. One of the most promising materials for use as the active medium in resistive memory is hafnia (HfO$_2$). However, an unresolved physics is the nature of defects and traps that are responsible for the charge transport in HRS state of resistive memory. In this study, we demonstrated experimentally and theoretically that oxygen vacancies are responsible for the HRS charge transport in resistive memory elements based on HfO$_2$. We also demonstrated that LRS transport occurs through a mechanism described according to percolation theory. Based on the model of multiphonon tunneling between traps, and assuming that the electron traps are oxygen vacancies, good quantitative agreement between the experimental and theoretical data of current-voltage characteristics were achieved. The thermal excitation energy of the traps in hafnia was determined based on the excitation spectrum and luminescence of the oxygen vacancies. The findings of this study demonstrate that in resistive memory elements using hafnia, the oxygen vacancies in hafnia play a key role in creating defects in HRS charge transport.",1309.0071v2 2020-09-26,Optical imaging of strain-mediated phase coexistence during electrothermal switching in a Mott insulator,"Resistive-switching -- the current-/voltage-induced electrical resistance change -- is at the core of memristive devices, which play an essential role in the emerging field of neuromorphic computing. This study is about resistive switching in a Mott-insulator, which undergoes a thermally driven metal-to-insulator transition. Two distinct switching mechanisms were reported for such a system: electric-field-driven resistive switching and electrothermal resistive switching. The latter results from an instability caused by Joule heating. Here, we present the visualization of the reversible resistive switching in a planar V$_2$O$_3$ thin-film device using high-resolution wide-field microscopy in combination with electric transport measurements. We investigate the interaction of the electrothermal instability with the strain-induced spontaneous phase-separation in the V$_2$O$_3$ thin film at the Mott-transition. The photomicrographs show the formation of a narrow metallic filament with a minimum width $\lesssim$ 500\,nm. Although the filament formation and the overall shape of the current-voltage characteristics (IVCs) are typical of an electrothermal breakdown, we also observe atypical effects like oblique filaments, filament splitting, and hysteretic IVCs with sawtooth-like jumps at high currents in the low-resistance regime. We were able to reproduce the experimental results in a numerical model based on a two-dimensional resistor network. This model demonstrates that resistive switching, in this case, is indeed electrothermal and that the intrinsic heterogeneity is responsible for the atypical effects. This heterogeneity is strongly influenced by strain, thereby establishing a link between switching dynamics and structural properties.",2009.12536v2 2023-10-01,Elucidating Dynamic Conductive State Changes in Amorphous Lithium Lanthanum Titanate for Resistive Switching Devices,"Exploration of novel resistive switching materials attracts attention to replace conventional Si-based transistors and to achieve neuromorphic computing that can surpass the limit of the current Von-Neumann computing for the time of Internet of Things (IoT). Materials priorly used to serve in batteries have demonstrated metal-insulator transitions upon an electrical biasing due to resulting compositional change. This property is desirable for future resistive switching devices. Amorphous lithium lanthanum titanate (a-LLTO) was originally developed as a solid-state electrolyte with relatively high lithium ionic conductivity and low electronic conductivity among oxide-type solid electrolytes. However, it has been suggested that electric conductivity of a-LLTO changes depending on oxygen content. In this work, the investigation of switching behavior of a-LLTO was conducted by employing a range of voltage sweep techniques, ultimately establishing a stable and optimal operating condition within the voltage window of -3.5 V to 3.5 V. This voltage range effectively balances the desirable trait of a substantial resistance change by three orders of magnitude with the imperative avoidance of LLTO decomposition. This switching behavior is also confirmed at nanodevice of Ni/LLTO/Ni through in-situ biasing inside focused-ion beam/scanning electron microscope (FIB-SEM). Experiment and computation with different LLTO composition shows that LLTO has two distinct conductivity states due to Ti reduction. The distribution of these two states is discussed using simplified binary model, implying the conductive filament growth during low resistance state. Consequently, our study deepens understanding of LLTO electronic properties and encourages the interdisciplinary application of battery materials for resistive switching devices.",2310.00543v1 2019-03-28,First Operation of a Resistive Shell Liquid Argon Time Projection Chamber -- A new Approach to Electric-Field Shaping,"We present a new technology for the shaping of the electric field in Time Projection Chambers (TPCs) using a carbon-loaded polyimide foil. This technology allows for the minimisation of passive material near the active volume of the TPC and thus is capable to reduce background events originating from radioactive decays or scattering on the material itself. Furthermore, the high and continuous electric resistivity of the foil limits the power dissipation per unit area and minimizes the risks of damages in the case of an electric field breakdown. Replacing the conventional field cage with a resistive plastic film structure called 'shell' decreases the number of components within the TPC and therefore reduces the potential points of failure when operating the detector. A prototype liquid argon (LAr) TPC with such a resistive shell and with a cathode made of the same material was successfully tested for long term operation with electric field values up to about 1.5 kV/cm. The experiment shows that it is feasible to successfully produce and shape the electric field in liquefied noble-gas detectors with this new technology.",1903.11858v2 2023-02-24,Antiferromagnetism of CeCd$_{0.67}$As$_{2}$ existing deep inside the narrow gap semiconducting state,"Single crystals of $R$Cd$_{0.67}$As$_2$ ($R$ = La and Ce) have been synthesized by high temperature ternary melt and their physical properties have been explored by means of magnetization, specific heat, electrical resistivity, Hall coefficient, and thermoelectric power measurements. $R$Cd$_{0.67}$As$_2$ compounds indicate a (structural) phase transition at high temperatures, accompanied by a remarkable increase of the electrical resistivity with an extremely low carrier concentration. CeCd$_{0.67}$As$_2$ exhibits a large magnetic anisotropy and an antiferromagnetic (AFM) order below $T_{N} = 4$~K. Magnetic susceptibility curves, together with magnetization isotherms and specific heat, are analyzed by the point charge model of crystalline electric field (CEF). In the paramagnetic state, the observed magnetic properties can be well explained by the CEF effects, implying that the 4$f$ moments remain localized. Electrical resistivity measurements, together with Hall resistivity and thermoelectric power, also suggest highly localized 4$f$ electrons, where Kondo contributions are negligible. The low temperature physical properties manifest strong magnetic field dependencies. For $H \perp c$, $T_{N}$ shifts to lower temperature as magnetic field increases, and eventually disappears at $H_{c} \sim 60$~ kOe. Inside the AFM state, three metamagnetic transitions are clearly evidenced from the magnetization isotherms. The RKKY interaction may be responsible for the AFM ordering in CeCd$_{0.67}$As$_2$, however it would have to be mediated by extremely low charge carriers. Although the AFM ordering temperature in CeCd$_{0.67}$As$_2$ can be continuously suppressed to zero, no AFM quantum phase transition is expected due to the lack of conduction electron clouds to screen the 4$f$ moments.",2302.12451v1 2003-05-06,High Magnetic Field Sensor Using LaSb2,"The magnetotransport properties of single crystals of the highly anisotropic layered metal LaSb2 are reported in magnetic fields up to 45 T with fields oriented both parallel and perpendicular to the layers. Below 10 K the perpendicular magnetoresistance of LaSb2} becomes temperature independent and is characterized by a 100-fold linear increase in resistance between 0 and 45 T with no evidence of quantum oscillations down to 50 mK. The Hall resistivity is hole-like and gives a high field carrier density of n ~ 3x10^20 cm^-3. The feasibility of using LaSb2 for magnetic field sensors is discussed.",0305116v1 2016-12-30,CdTe and CdZnTe Crystal Growth and Production of Gamma Radiation Detectors,"Bridgman CdTe and CdZnTe crystal growth, with cadmium vapor pressure control, is applied to production of semiconductor gamma radiation detectors. Crystals are highly donor doped and highly electrically conducting. Annealing in tellurium vapors transforms them into a highly compensated state of high electrical resistance and high sensitivity to gamma radiation. N-type detectors, equipped with ohmic contacts, and a grounded guard ring around the positive contact, are not sensitive to hole trapping. Conductivity control, by the doping level, optimizes the detector operation by trade-off between electrons' lifetime and electrical resistance. Gamma spectra of single detectors and detector arrays are presented. Detector optimization and gamma detection mechanisms are discussed.",1612.09571v1 2015-06-25,Metallic multilayers for X-band Bragg reflector applications,"We present a structural and high frequency (8.72GHz) electrical characterization of sputter deposited Ti/W, Ti/Ru and Mo/Ti metallic multilayers for potential application as acoustic Bragg reflectors. We prove that all metallic multilayers comprised of different acoustic impedance metals such as Ti, W, Mo are promising candidates for Bragg reflector/bottom electrode in full X-band thin film acoustic resonators. Values for high frequency resistivity of the order of $10^{-8} ohm.m$ are measured by use of a contact-free/non-invasive sheet resistance method.",1506.07702v1 2014-06-11,Very high thermoelectric power factor in a Fe3O4/SiO2/p-type Si(100)heterostructure,"The thermoelectric and transport properties of a Fe3O4/SiO2/p-Si(100) heterostructure have been investigated between 100 and 300 K. Both Hall and Seebeck coefficients change sign from negative to positive with increasing temperature while the resistivity drops sharply due to tunneling of carriers into the p-Si(100). The low resistivity and large Seebeck coefficient of Si give a very high thermoelectric power factor of 25.5mW/K2m at 260K which is an underestimated, lower limit value and is related to the density of states and difference in the work functions of Fe3O4 and Si(100) that create an accumulation of majority holes at the p-Si/SiO2 interface",1406.2814v1 2002-10-10,Effects of Pressure on Electron Transport and Local Structure of Manganites: Low to High Pressure Regime,"The pressure dependence of the resistivity and structure of La0.60Y0.07Ca0.33MnO3 has been explored in the pressure range from 1 atm to ~7 GPa. The metal to insulator transition temperature (TMI) was found to reach a maximum and the resistivity achieves a minimum at ~3.8 GPa. Beyond this pressure, TMI is reduced with a concomitant increase in the resistivity. Structural measurements at room temperature show that at low pressure (below 2 GPa) the Mn-O bond lengths are compressed. Between ~2 and ~4 GPa, a pressure induced enhancement of the Jahn-Teller (JT) distortion occurs in parallel with an increase in Mn-O1-Mn bond angle to ~180 (degree). Above ~4 GPa, the Mn-O1-Mn bond angle is reduced while the JT distortion appears to remain unchanged. The resistivity above TMI is well modeled by variable range hopping. The pressure dependence of the localization length follows the behavior of TMI.",0210220v2 2003-07-31,Is Room Temperature Superconductivity in Carbon Nanotubes Too Wonderful to Believe?,"It is well known that copper-based perovskite oxides rightly enjoy consensus as high-temperature superconductors on the basis of two signatures: Meissner effect and zero resistance. In contrast, I provide over twenty signatures for room temperature superconductivity in carbon nanotubes. The one-dimensionality of the nanotubes complicates the right-of-passage for prospective quasi-one-dimensional superconductors. The Meissner effect is less visible because the diameters of nanotubes are much smaller than the penetration depth. Zero resistance is less obvious because of the quantum contact resistance and significant quantum phase slip, both of which are associated with a finite number of transverse conduction channels. Nonetheless, on-tube resistance at room temperature has been found to be indistinguishable from zero for many individual multi-walled nanotubes. On the basis of more than twenty arguments, I suggest that carbon nanotubes deserve to be classified as room temperature superconductors. The mechanism for room-temperature superconductivity may arise from strong electron-phonon and electron-plasmon coupling.",0307770v3 2003-09-24,High critical fields in MgB2 thin films with various resistivity values,"In this paper, we analyze the upper critical field of four MgB2 thin films, with different resistivity (between 5 to 50 mWcm) and critical temperature (between 29.5 to 38.8 K), measured up to 28 Tesla. In the perpendicular direction the critical fields vary from 13 to 24 T and we can estimate 42-57 T range in other direction. We observe linear temperature dependence even at low temperatures without saturation, in contrast to BCS theory. Considering the multiband nature of the superconductivity in MgB2, we conclude that two different scattering mechanisms influence separately resistivity and critical field. In this framework, resistivity values have been calculated from Hc2(T) curves and compared with the measured ones.",0309543v1 2004-11-18,Hysteretic current-voltage characteristics and resistance switching at an epitaxial oxide Schottky junction SrRuO$_{3}$/SrTi$_{0.99}$Nb$_{0.01}$O$_{3}$,"Transport properties have been studied for a perovskite heterojunction consisting of SrRuO$_{3}$ (SRO) film epitaxially grown on SrTi$_{0.99}$Nb$_{0.01}$O$_{3}$ (Nb:STO) substrate. The SRO/Nb:STO interface exhibits rectifying current-voltage ($I$-$V$) characteristics agreeing with those of a Schottky junction composed of a deep work-function metal (SRO) and an $n$-type semiconductor (Nb:STO). A hysteresis appears in the $I$-$V$ characteristics, where high resistance and low resistance states are induced by reverse and forward bias stresses, respectively. The resistance switching is also triggered by applying short voltage pulses of 1 $\mu$s - 10 ms duration.",0411474v1 2005-09-13,Evidence for High-Temperature Superconductivity in Doped Laser-Processed Sr-Ru-O,"We have discovered that samples of a new material produced by special processing of crystals of Sr2RuO4 (which is known to be a triplet superconductor with Tc values ~1.0-1.5K) exhibit signatures of superconductivity (zero DC resistance and expulsion of magnetic flux) at temperatures exceeding 200K. The special processing includes deposition of a silver coating and laser micromachining; Ag doping and enhanced oxygen are observed in the resultant surface layer. The transition, whether measured resistively or by magnetic field expulsion, is broad. When the transition is registered by resistive methods, the critical temperature is markedly reduced when the measuring current is increased. The resistance disappears by about 190K. The highest value of Tc registered by magneto-optical visualization is about 220K and even higher values (up to 250K) are indicated from the SQUID-magnetometer measurements.",0509313v1 2006-05-04,Threshold Resistance in the DC Josephson Effect,"We show that SIS Josephson junctions have a threshold resistance, above which the Josephson coupling and the supercurrents become extremely small, due to the shrinking of the Cooper pair size during the Josephson tunneling. Accordingly, the threshold resistance is smaller for higher Tc superconductors with small Cooper pair size and for the insulating barrier with higher resistance. This understanding agrees with the observations in SIS junctions of low Tc superconductors, such as Sn, Pb, and Nb. For MgB2 it explains why the big gap does not show the supercurrents, unlike the small gap. Furthermore, it is consistent with the fact that high Tc cuprates show the Josephson effects only for SNS type junctions, including the intrinsic Josephson effects.",0605122v1 2007-04-03,Scaling of Resistance and Electron Mean Free Path of Single-Walled Carbon Nanotubes,"We present an experimental investigation on the scaling of resistance in individual single walled carbon nanotube devices with channel lengths that vary four orders of magnitude on the same sample. The electron mean free path is obtained from the linear scaling of resistance with length at various temperatures. The low temperature mean free path is determined by impurity scattering, while at high temperature the mean free path decreases with increasing temperature, indicating that it is limited by electron-phonon scattering. An unusually long mean free path at room temperature has been experimentally confirmed. Exponentially increasing resistance with length at extremely long length scales suggests anomalous localization effects.",0704.0300v2 2007-09-12,Thermal Transient Characterization of Packaged Thin Film Microcoolers,"A network identification by deconvolution (NID) method is applied to the thermal transient response of packaged and unpackaged microcoolers. A thin film resistor on top of the device is used as the heat source and the temperature sensor. The package and the bonding thermal resistances can be easily identified by comparing structure functions. High-speed coplanar probes are used to achieve a short time resolution of roughly 100ns in the transient temperature response. This is used to separate the thermal properties of the thin film from the substrate. The obtained thermal resistances of the buffer layer and Silicon substrate are consistent with the theoretical calculations. In order to estimate the superlattice thermal resistance and separate it from the thin SiNx layer deposited underneath the thin film resistive sensor, an order of magnitude faster thermal transient response is needed.",0709.1817v1 2007-12-09,Interplay between carrier localization and magnetism in diluted magnetic and ferromagnetic semiconductors,"The presence of localized spins exerts a strong influence on quantum localization in doped semiconductors. At the same time carrier-mediated interactions between the localized spins are modified or even halted by carriers' localization. The interplay of these effects is discussed for II-VI and III-V diluted magnetic semiconductors. This insight is exploited to interpret the complex dependence of resistance on temperature, magnetic field, and concentration of valence-band holes in (Ga,Mn)As. In particular, high field negative magnetoresistance results from the orbital weak localization effect. The resistance maximum and the associated negative magnetoresistance near the Curie temperature are assigned to the destructive influence of preformed ferromagnetic bubbles on the ""antilocalization"" effect driven by disorder-modified carrier-carrier interactions. These interactions account also for the low-temperature increase of resistance. Furthermore, the sensitivity of conductance to spin splitting and to scattering by spin disorder may explain resistance anomalies at coercive fields, where relative directions of external and molecular fields change.",0712.1293v2 2009-08-25,Bipolar resistive switching in amorphous titanium oxide thin films,"Using isothermal and temperature-dependent electrical measurements, we investigated the resistive switching mechanism of amorphous titanium oxide thin films deposited by a plasma-enhanced atomic layer deposition method between two aluminum electrodes. We found a bipolar resistive switching behavior in the high temperature region (> 140 K), and two activation energies of shallow traps, 0.055 eV and 0.126 eV in the ohmic current regime. We also proposed that the bipolar resistive switching of amorphous TiO2 thin films is governed by the transition of conduction mode from a bulk-limited SCLC model (Off state) to an interface-limited Schottky emission (On state), generated by the ionic movement of oxygen vacancies.",0908.3525v1 2009-12-09,Scaling Properties of Ge-SixGe1-x Core-Shell Nanowire Field Effect Transistors,"We demonstrate the fabrication of high-performance Ge-SixGe1-x core-shell nanowire field-effect transistors with highly doped source and drain, and systematically investigate their scaling properties. Highly doped source and drain regions are realized by low energy boron implantation, which enables efficient carrier injection with a contact resistance much lower than the nanowire resistance. We extract key device parameters, such as intrinsic channel resistance, carrier mobility, effective channel length, and external contact resistance, as well as benchmark the device switching speed and ON/OFF current ratio.",0912.1827v1 2010-07-21,The effects of superconductor-stabilizer interfacial resistance on quench of a pancake coil made out of coated conductor,"We present the results of numerical analysis of normal zone propagation in a stack of $YBa_2Cu_3O_{7-x}$ coated conductors which imitates a pancake coil. Our main purpose is to determine whether the quench protection quality of such coils can be substantially improved by increased contact resistance between the superconducting film and the stabilizer. We show that with increased contact resistance the speed of normal zone propagation increases, the detection of a normal zone inside the coil becomes possible earlier, when the peak temperature inside the normal zone is lower, and stability margins shrink. Thus, increasing contact resistance may become a viable option for improving the prospects of coated conductors for high $T_c$ magnets applications.",1007.3768v2 2012-10-15,Bi2Te_xSe_y series studied by resistivity and thermopower,"We study the detailed temperature and composition dependence of the resistivity, $\rho(T)$, and thermopower, $S(T)$, for a series of layered bismuth chalcogenides Bi$_2$Te$_{3-x}$Se$_x$, and report the stoichiometry dependence of the optical band gap. In the resistivity of the most compensated member, Bi$_2$Te$_{2.1}$Se$_{0.9}$, we find a low-temperature plateau whose onset temperature correlates with the high-temperature activation energy. For the whole series $S(T)$ can be described by a simple model for an extrinsic semiconductor. By substituting Se for Te, the Fermi level is tuned from the valence band into the conduction band. The maximum values of $S(T)$, bulk band gap as well the activation energy in the resistivity are found for $x \approx 0.9$.",1210.3901v3 2014-07-14,Multistate nonvolatile straintronics controlled by a lateral electric field,"We present a multifunctional and multistate permanent memory device based on lateral electric field control of a strained surface. Sub-coercive electrical writing of a remnant strain of a PZT substrate imprints stable and rewritable resistance changes on a CoFe overlayer. A proof-of-principle device, with the simplest resistance strain gage design, is shown as a memory cell exhibiting 17-memory states of high reproducibility and reliability for nonvolatile operations. Magnetoresistance of the film also depends on the cell state, and indicates a rewritable change of magnetic properties persisting in the remnant strain of the substrate. This makes it possible to combine strain, magnetic and resistive functionalities in a single memory element, and suggests that sub-coercive stress studies are of interest for straintronics applications.",1407.3651v2 2015-10-29,"Resistive superconducting transition and effects of atmospheric exposure in the intercalation superconductor Ax(C2H8N2)yFe2-zSe2 (A = Li, Na)","We have succeeded in observing zero-resistivity in newly discovered intercalation superconductors Ax(C2H8N2)yFe2-zSe2 (A = Li, Na) with Tc = 45 K, using the sintered pellet samples. The electrical resistivity, \r{ho}, in the normal state is metallic and Tconset defined in the $\rho$ measurements, is as high as ~ 57 K. We have also investigated effects of the atmospheric exposure in Lix(C2H8N2)yFe2-zSe2. It has been found that both the crystal structure and superconductivity are maintained at least up to several days, indicating this material is comparatively resistant to the atmospheric exposure.",1510.08629v1 2016-05-19,Resistive Switching Characteristics of Al/Si3N4/p-Si MIS-Based Resistive Switching Memory Devices,"In this study, we proposed and demonstrated a self-rectifying property of silicon nitride (Si3N4)-based resistive random access memory device by employing p-type silicon (p-Si) as bottom electrode. The RRAM devices consisted of Al/Si3N4/p-Si are fabricated by a low presure chemical vapor deposition and exhibited an intrinsic diode property with non-linear current-voltage (I-V) behavior. In addition, compared to conventional metal/insulator/metal (MIM) structure of Al/Si3N4/Ti RRAM cells, operating current in whole bias regions for proposed metal/insulator/semiconductor (MIS) cells has been dramatically lowered because introduced p-Si bottom electrode efficiently suppresses the current in both low and high resistive states. As a result, the results mean that by employing p-Si as bottom electrode the Si3N4-based RRAM cells can be applied to selector-free RRAM cells.",1605.06006v1 2016-06-25,Transport mechanism through metal-cobaltite interfaces,"The resistive switching (RS) properties as a function of temperature were studied for Ag/La$_{1-x}$Sr$_x$CoO$_3$ (LSCO) interfaces. The LSCO is a fully-relaxed 100 nm film grown by metal organic deposition on a LaAlO$_3$ substrate. Both low and a high resistance states were set at room temperature and the temperature dependence of their current-voltage (IV) characteristics was mea- sured taking care to avoid a significant change of the resistance state. The obtained non-trivial IV curves of each state were well reproduced by a circuit model which includes a Poole-Frenkel element and two ohmic resistances. A microscopic description of the changes produced by the RS is given, which enables to envision a picture of the interface as an area where conductive and insulating phases are mixed, producing Maxwell-Wagner contributions to the dielectric properties.",1606.07974v1 2016-07-19,Non-quasiparticle transport and resistivity saturation: A view from the large-N limit,"The electron dynamics in metals are usually well described by the semiclassical approximation for long-lived quasiparticles. However, in some metals, the scattering rate of the electrons at elevated temperatures becomes comparable to the Fermi energy; then, this approximation breaks down, and the full quantum-mechanical nature of the electrons must be considered. In this work, we study a solvable, large-$N$ electron-phonon model, which at high temperatures enters the non-quasiparticle regime. In this regime, the model exhibits ""resistivity saturation"" to a temperature-independent value of the order of the quantum of resistivity - the first analytically tractable model to do so. The saturation is not due to a fundamental limit on the electron lifetime, but rather to the appearance of a second conductivity channel. This is suggestive of the phenomenological ""parallel resistor formula"", known to describe the resistivity of a variety of saturating metals.",1607.05725v1 2016-11-04,Origin of multistate resistive switching in Ti/manganite/Si$O_x$/Si heterostructures,"We report on the growth and characterization of Ti/$La_{1/3}$$Ca_{2/3}$Mn$O_3$/Si$O_x$/n-Si memristive devices. We demonstrate that using current as electrical stimulus unveils an intermediate resistance state, in addition to the usual high and low resistance states that are observed in standard voltage controlled experiments. Based on thorough electrical characterization (impedance spectroscopy, current-voltage curves analysis), we disclose the contribution of three different microscopic regions of the device to the transport properties: an ohmic incomplete metallic filament, a thin manganite layer below the filament tip exhibiting Poole-Frenkel like conduction, and the SiOx layer with an electrical response well characterized by a Child-Langmuir law. Our results suggest that the existence of the SiOx layer plays a key role in the stabilization of the intermediate resistance level, indicating that the combination of two or more active RS oxides adds functionalities in relation to single-oxide devices. We understand that these multilevel devices are interesting and promising as their fabrication procedure is rather simple and they are fully compatible with standard Si-based electronics.",1611.01552v2 2017-06-07,Spatially Resolved Thermometry of Resistive Memory Devices,"The operation of resistive and phase-change memory (RRAM and PCM) is controlled by highly localized self-heating effects, yet detailed studies of their temperature are rare due to challenges of nanoscale thermometry. Here we show that the combination of Raman thermometry and scanning thermal microscopy (SThM) can enable such measurements with high spatial resolution. We report temperature-dependent Raman spectra of HfO$_2$, TiO$_2$ and Ge$_2$Sb$_2$Te$_5$ (GST) films, and demonstrate direct measurements of temperature profiles in lateral PCM devices. Our measurements reveal that electrical and thermal interfaces dominate the operation of such devices, uncovering a thermal boundary resistance of 30 m$^2$K$^{-1}$GW$^{-1}$ at GST-SiO$_2$ interfaces and an effective thermopower 350 $\mu$V/K at GST-Pt interfaces. We also discuss possible pathways to apply Raman thermometry and SThM techniques to nanoscale and vertical resistive memory devices.",1706.02318v1 2017-12-03,Microstructure and properties of Cu-Sn-Zn-TiO2 Nano-composite coatings on mild steel,"Cu-Sn-Zn coatings have been widely used in industry for their unique properties, such as good conductivity, high corrosion resistance and excellent solderability. To further improve the mechanical performance of Cu-Sn-Zn coatings, powder-enhanced method was applied in the current study and Cu-Sn-Zn-TiO2 nano-composite coatings with different TiO2 concentration were fabricated. The microstructure of Cu-Sn-Zn-TiO2 nano-composite coatings were investigated by X-ray diffraction (XRD) and Scanning Electron Microscopy (SEM). The mechanical properties of coatings including microhardness and wear resistance were studied. The results indicate that the incorporation of TiO2 nanoparticle can significantly influence the properties of Cu-Sn-Zn coatings. The microhardness of Cu-Sn-Zn coating was increased to 383 HV from 330 HV with 1g/L TiO2 addition. Also, the corrosion resistance of coating was enhanced. The effects of TiO2 nanoparticle concentration on the microstructure, mechanical properties and corrosion resistance of Cu-Sn-Zn-TiO2 nano-composite coatings were discussed.",1712.00853v1 2022-02-11,Comparison of the charge-crystal and charge-glass state in geometrically frustrated organic conductors studied by fluctuation spectroscopy,"We present a systematic investigation of the low-frequency charge carrier dynamics in different charge states of the organic conductors $\theta$-(BEDT-TTF)$_2$$M$Zn(SCN)$_4$ with $M$=Rb,Tl, which result from quenching or relaxing the charge degrees of freedom on a geometrically frustrated triangular lattice. Due to strong electronic correlations these materials exhibit a charge-ordering transition, which can be kinetically avoided by rapid cooling resulting in a so-called charge-glass state without long-range order. The combination of fluctuation spectroscopy and a heat pulse method allows us to study and compare the resistance fluctuations in the low-resistive quenched and the high-resistive charge-ordered state, revealing striking differences in the respective noise magnitudes. For both compounds, we find strongly enhanced resistance fluctuations right at the metal-insulator transition and a broad noise maximum in the slowly cooled charge-crystal state with partly dominating two-level processes revealing characteristic activation energies.",2202.05602v1 2007-10-09,Strong reduction of field-dependent microwave surface resistance in YBa$_{2}$Cu$_{3}$O$_{7-δ}$ with sub-micrometric BaZrO$_3$ inclusions,"We observe a strong reduction of the field induced thin film surface resistance measured at high microwave frequency ($\nu=$47.7 GHz) in YBa$_{2}$Cu$_{3}$O$_{7-\delta}$ thin films grown on SrTiO$_3$ substrates, as a consequence of the introduction of sub-micrometric BaZrO$_3$ particles. The field increase of the surface resistance is smaller by a factor of $\sim$3 in the film with BaZrO$_3$ inclusions, while the zero-field properties are not much affected. Combining surface resistance and surface reactance data we conclude (a) that BaZrO$_3$ inclusions determine very deep and steep pinning wells and (b) that the pinning changes nature with respect to the pure film.",0710.1754v1 2017-08-04,Tunable Spin-Orbit Torques in Cu-Ta Binary Alloy Heterostructures,"The spin Hall effect (SHE) is found to be strong in heavy transition metals (HM), such as Ta and W, in their amorphous and/or high resistivity form. In this work, we show that by employing a Cu-Ta binary alloy as buffer layer in an amorphous Cu$_{100-x}$Ta$_{x}$-based magnetic heterostructure with perpendicular magnetic anisotropy (PMA), the SHE-induced damping-like spin-orbit torque (DL-SOT) efficiency $|\xi_{DL}|$ can be linearly tuned by adjusting the buffer layer resistivity. Current-induced SOT switching can also be achieved in these Cu$_{100-x}$Ta$_{x}$-based magnetic heterostructures, and we find the switching behavior better explained by a SOT-assisted domain wall propagation picture. Through systematic studies on Cu$_{100-x}$Ta$_{x}$-based samples with various compositions, we determine the lower bound of spin Hall conductivity $|\sigma_{SH}|\approx2.02\times10^{4}[\hbar/2e]\Omega^{-1}\cdot\operatorname{m}^{-1}$ in the Ta-rich regime. Based on the idea of resistivity tuning, we further demonstrate that $|\xi_{DL}|$ can be enhanced from 0.087 for pure Ta to 0.152 by employing a resistive TaN buffer layer.",1708.01356v1 2019-03-29,Effect of synthesis conditions on the electrical resistivity of TiSe$_2$,"Dilute impurities and growth conditions can drastically affect the transport properties of TiSe$_2$, especially below the charge density wave transition. In this paper, we discuss the effects of cooling rate, annealing time and annealing temperature on the transport properties of TiSe$_2$: slow cooling of polycrystalline TiSe$_2$ post-synthesis drastically increases the low temperature resistivity, which is in contrast to the metallic behavior of single-crystalline TiSe$_2$ due to charge doping from the residual iodine transport agent. A logarithmic increase of resistivity upon cooling and negative magnetoresistance with a sharp cusp around zero field are observed for the first time for the polycrystalline TiSe$_2$ samples, pointing to weak-localization effects due to low dimensionality. Annealing at low temperatures has a similar, but less drastic effect. Furthermore, rapid quenching of the polycrystalline samples from high temperatures freezes in disorder, leading to a decrease in the low temperature resistivity.",1903.12375v3 2019-12-18,A theory of resistivity in Kondo lattice materials: the memory function approach,"We theoretically analyse D.C. resistivity($\rho$) in the Kondo-lattice model using the powerful memory function approach. The complete temperature evolution of $\rho$ is investigated using the W\""{o}lfle-G\""{o}tze expansion of the memory function. The resistivity in this model originates due to spin-flip magnetic scattering of conduction $s$-electron off the quasi-localized $d$ or $f$ electron spins. We find the famous resistivity upturn at lower temperature regime ($k_B T<<\mu_d$), where $\mu_d$ is the effective chemical potential of $d$-electrons. In the high temperature regime $(\mu_d< 14 000 switchings) a prospective of use for synthesized Ti/TiO2-NT/Au micromemristors with oxide layer thickness of 160 nm in non-volatile memory is shown. Keywords: anodic titania, titanium dioxide nanotubes, nanotubular structure, memristor, resistive switching",1906.06555v1 2019-11-28,Tailored joint fabrication process derived ultra-low resistance MgB2 superconducting joint,"We report an ultra-low resistance superconducting joint using unreacted multifilament MgB2 wires produced by tailoring the powder compaction pressure within the joint with heat treatment conditions. The joint demonstrated an ultra-low resistance of 5.48 x 10^-15 ohms and critical current (Ic) of 91.3 A at 20 K in self-field. The microstructural and composition studies of the joint revealed cracks and a high amount of MgO, respectively. These two features reduced the Ic of the joint to some extent; nevertheless, the joint resistance was not affected by it. Our tailored joining process will play a pivotal role in superconducting joint development.",1911.12645v1 2020-10-23,Improvement of HRS Variability in OxRRAM by Tailored Metallic Liner,"In this work, we propose a novel integration in order to significantly reduce the High Resistance State vari-ability and to improve thermal stability in Oxide-based Resistive Random Access Memory (OxRRAM) devices. A novel device featuring a metallic liner, acting as a parallel resistance, is presented. To assess the effect of this solution, we compare the results with a standard OxRRAM cell structure. A very good stability of the resistive states, both in endurance and temperature, is highlighted and explained thanks to a conductive fila-ment based model.",2010.12210v1 2020-11-01,Light induced resistive switching in copper oxide thin films,"Copper oxide thin film based metal-insulator-metal structures were subjected to white light irradiation.The top electrodes included Al, Cr and Ni while the bottom electrode was either Au or Pt. A white light pulse controls the set process and this light induced set (LIS) can be performed at very low voltages (tens of milli volts) which is not possible in the normal set process. The LIS is initiated at the positive edge of the pulse and there is no effect of the falling edge of the light. In most cases the high resistance state (HRS) to low resistance state (LRS) transition is irreversible i.e.the devices continue to remain in the LRS even after the light pulse is switched off. Light induced reset (LIR) is achieved in only one device structure Al/CuxO/Au. By using LIS and LIR, set and reset power of the device can be reduced to a great extent and the set and reset parameters variation also reduces. The current work, thus, points to the possibility of formation and compliance-free resistive random access memory devices.",2011.00423v1 2021-04-05,Charge density wave and finite-temperature transport in minimally twisted bilayer graphene,"We study phenomena driven by electron-electron interactions in the minimally twisted bilayer graphene (mTBLG) with a perpendicular electric field. The low-energy degrees of freedom in mTBLG are governed by a network of one-dimensional domain-wall states, described by two channels of one-dimensional linearly dispersing spin-1/2 fermions. We show that the interaction can realize a spin-gapped inter-channel charge density wave (CDW) state at low temperatures, forming a ""Coulomb drag"" between the channels and leaving only one charge conducting mode. For sufficiently high temperatures, power-law-in-temperature resistivity emerges from the charge umklapp scatterings within a domain wall. Remarkably, the presence of the CDW states can strengthen the charge umklapp scattering and induce a resistivity minimum at an intermediate temperature corresponding to the CDW correlation energy. We further discuss the conditions that resistivity of the network is dominated by the domain walls. In particular, the power-law-in-temperature resistivity results can apply to other systems that manifest topological domain-wall structures.",2104.02084v2 2021-05-14,Mechanical Response of Mesoporous Amorphous NiTi Alloy to External Deformations,"The porous titanium nickelide is very popular in various industries due to unique combination of physical and mechanical properties such as shape memory effect, high corrosion resistance, and biocompatibility. The non-equilibrium molecular dynamics simulation was applied to study the influence of porosity degree on mechanical properties of porous amorphous titanium nickelide at uniaxial tension, uniaxial compression, and uniform shear. We have found that the porous amorphous alloy is characterized by a relatively large value of Young's modulus in comparison to its crystalline analogue. It has been found that the system with a percolated network of pores exhibits improved elastic characteristics associated with resistance to tensile and shear. The system contained isolated spherical pores is more resistant to compression and less resistant to tensile and shear. These results can be applied to develop and improve the methods for making amorphous metal foams.",2105.06693v1 2021-08-01,Sb concentration dependent Structural and Transport properties of Polycrystalline (Bi1-xSbx)2Te3 Mixed crystal,"(Bi1-xSbx)2Te3 (x=0.60, 0.65, 0.68, 0.70, 0.75 and 0.80) mixed crystals have been synthesized by solid state reaction. In depth structural, thermal, transport and electronic properties are reported. Defect and disorder play a crucial role in structural and transport behaviour. Disorder induced iso-structural phase transition is observed at x=0.70, which is supported by the structural and transport properties data. Debye temperature has been estimated from the powder diffraction data. Differential scanning calorimetry (DSC) data confirms the glass transition in the material. Low temperature resistivity data shows Variable range hopping mechanism whereas high temperature data follows activated behaviour. Activation energy is calculated from the semiconducting region of resistivity data. Both Hall measurement and temperature dependent thermopower data (S(T)) confirms that samples are p-type in nature. Density of state effective mass has been estimated from Pisarenko relation and corroborated with resistivity data. Thermal conductivity (k) is estimated using experimentally obtained data. Figure of Merit (ZT) of the synthesized samples are calculated using resistivity, S(T) and k. Structural and transport properties are correlated, confirms the transition from disorder to order state. Defect and disorder are corroborated with structural and Thermoelectric properties of the synthesized samples.",2108.00525v1 2021-10-16,Topological phonons in an inhomogeneously strained silicon-6: Possible evidence of the high temperature spin superfluidity and the second sound of topological phonons,"The superposition of topological phonons and flexoelectronic charge separation in an inhomogeneously strain Si give rise to topological electronic magnetism of phonons. The topological electronic magnetism of phonons is also expected to give rise to stationary spin current or spin superfluidity. In this experimental study, we present possible evidence of spin superfluidity in an inhomogeneously strained p-Si thin films samples. The spin superfluidity is uncovered using non-local resistance measurement. A resonance behavior is observed in a non-local resistance measurement at 10 kHz and between 270 K and 281.55 K, which is attributed to the second sound. The observation of second sound and spatially varying non-local resistance phase are the evidences for spin superfluidity. The spatially varying non-local resistance with opposite phase are also observed in Pt/MgO/p-Si sample. The overall non-local responses can be treated as a standing waveform from temporal magnetic moments of the topological phonons.",2110.08431v1 2021-12-10,"Transport in the emergent Bose liquid: Bad metal, strange metal, and weak insulator, all in one system","Non-saturating high-temperature resistivity (""bad metal""), T-linear low-temperature resistivity (""strange metal""), and a crossover to activation-free growth of the resistivity in the low-temperature limit (""weak insulator"") are among the most exotic behaviors widely observed in many strongly correlated materials for decades that defy the standard Fermi liquid description of solids. Here we investigate these puzzling behaviors by computing temperature-dependent optical conductivity of an emergent Bose liquid and find that it reproduces all the unexplained features of the experiments, including a featureless continuum and a well-known mid-infrared peak. Amazingly and with physically intuitive mechanisms, the corresponding doping- and temperature-dependent resistivity displays the bad metal and strange metal simultaneously and sometimes weak insulating behaviors as well. The unification of all these non-Fermi liquid behaviors in a single model suggests that a new quantum state of matter, namely the emergent Bose liquid, will guide the development of the next generation of solid state physics.",2112.05747v1 2022-04-20,Electrical breakdown in Thick-GEM based WELL detectors,"The occurrence of electrical discharges in gas detectors restricts their dynamic range and degrades their performance. Among the different methods developed to mitigate discharge effects, the use of resistive materials in the detector assembly was found to be very effective. In this work, we present the results of a comparative study of electrical discharges in Thick-GEM-based WELL-type detectors - with and without resistive elements. We present a new method to measure discharges in the resistive-detector configurations; it allows demonstrating, for the first time, the occurrence of discharges also in the Resistive-Plate WELL detector configuration. It also provides direct evidence for the Raether limit.",2204.09445v2 2022-11-27,Evolution of Resistive Switching Characteristics in WO3-x-based MIM Devices by Tailoring Oxygen Deficiency,"We report on resistive switching (RS) characteristics of W/WO3-x/Pt-based thin film memristors modulated by precisely controlled oxygen non-stoichiometry. RS properties of the devices with varied oxygen vacancy (VO) concentration have been studied by measuring their DC current voltage properties. Switchability of the resistance states in the memristors have been found to depend strongly on the VOs concentration in the WO3-x layer. Depending on x, the memristors exhibited forming-free bipolar, forming-required bipolar and non-formable characteristics. Devices with high VOs concentration (~1*1021 cm-3) exhibited lower initial resistance and memory window of only 15, which has been increased to ~6500 with reducing VOs concentration to ~5.8*1020 cm-3. Forming-free, stable RS with memory window of ~2000 have been realized for a memristor possessing VOs concentration of ~6.2*1020 cm-3. Investigation of the conduction mechanism suggests that tailoring VOs concentration modifies the formation and dimension of the conducting filaments as well as the Schottky barrier height at WO3-x/Pt interface which deterministically modulates RS characteristics of the WO3-x based memristors.",2211.14809v1 2024-05-13,Durability of MgO/hydromagnesite mortars -- Resistance to chlorides and corrosion,"The durability of MgO/hydromagnesite mortars was studied with respect to their corrosion performance and resistance to chloride attack and moisture. MgO/hydromagnesite pastes were cured in chloride solution to induce potential formation of Mg-chlorides; however, no such phases were observed. Rapid chloride ingress measurements demonstrated high penetration resistance and low chloride migration coefficients, i.e. D_Cl = 1e-13 to 1e-12 m^2/s. The corrosion rate of carbon steel embedded in MgO/HY mortars, as determined by linear polarization resistance measurements, was in the range icorr = 1e-9 A/cm^2 in dry and 1e-7 A/cm^2 in wet conditions, irrespective of the mortar composition or curing condition.These findings corroborate the hypothesis that, in the absence of chlorides, the moisture condition is the primary predictor of corrosion rate of carbon steel in the MgO/hydromagnesite binder. These accelerated, short-term experiments suggest that the binder may be suited to protect embedded carbon steel from corrosion under specific exposure conditions of practical relevance.",2405.08164v1 2024-05-27,Electronic thermal resistivity and quasi-particle collision cross-section in semi-metals,"Electron-electron collisions lead to a T-square component in the electrical resistivity of Fermi liquids. The case of liquid $^3$He illustrates that the \textit{thermal} resitivity of a Fermi liquid has a T-square term, expressed in m$\cdot$W$^{-1}$. Its natural units are $\hbar/k_FE_F^2$. Here, we present a high-resolution study of the thermal conductivity in bismuth, employing magnetic field to extract the tiny electronic component of the total thermal conductivity and resolving signals as small as $\approx 60 \mu$K. We find that the electronic thermal resistivity follows a T-square temperature dependence with a prefactor twice larger than the electric T-square prefactor. Adding this information to what has been known for other semi-metals, we find that the prefactor of the T-square thermal resistivity scales with the square of the inverse of the Fermi temperature, implying that the dimensionless fermion-fermion collision cross-section is roughly proportional to the Fermi wavelength, indicating that it is not simply set by the strength of the Coulomb interaction.",2405.16984v2 2017-10-02,Anomalous magnetotransport properties of high-quality single crystals of Weyl semimetal WTe2: Sign change of Hall resistivity,"We report on a systematic study of Hall effect using high quality single crystals of type-II Weyl semimetal WTe2 with the applied magnetic field B//c. The residual resistivity ratio of 1330 and the large magnetoresistance of 1.5\times10^6 % in 9 T at 2 K, being in the highest class in the literature, attest to their high quality. Based on a simple two-band model, the densities (n_e and n_h) and mobilities (\mu_e and \mu_h) for electron and hole carriers have been uniquely determined combining both Hall- and electrical-resistivity data. The difference between ne and nh is ~1% at 2 K, indicating that the system is in an almost compensated condition. The negative Hall resistivity growing rapidly below ~20 K is due to a rapidly increasing \mu_h/\mu_e approaching one. Below 3 K in a low field region, we found the Hall resistivity becomes positive, reflecting that \mu_h/\mu_e finally exceeds one in this region. These anomalous behaviors of the carrier densities and mobilities might be associated with the existence of a Lifshitz transition and/or the spin texture on the Fermi surface.",1710.00570v1 2021-10-14,Superconductor-insulator transitions in three-dimensional indium-oxide at high pressures,"Experiments investigating magnetic-field-tuned superconductor-insulator transition (HSIT) mostly focus on two-dimensional material systems where the transition and its proximate ground-state phases, often exhibit features that are seemingly at odds with the expected behavior. Here we present a complementary study of a three-dimensional pressure-packed amorphous indium-oxide (InOx) powder where granularity controls the HSIT. Above a low threshold pressure of ~0.2 GPa, vestiges of superconductivity are detected, although neither a true superconducting transition nor insulating behavior are observed. Instead, a saturation at very high resistivity at low pressure is followed by saturation at very low resistivity at higher pressure. We identify both as different manifestations of anomalous metallic phases dominated by superconducting fluctuations. By analogy with previous identification of the low resistance saturation as a ""failed superconductor"", our data suggests that the very high resistance saturation is a manifestation of a ""failed insulator"". Above a threshold pressure of ~6 GPa, the sample becomes fully packed, and superconductivity is robust, with TC tunable with pressure. A quantum critical point at PC~25 GPa marks the complete suppression of superconductivity. For a finite pressure below PC, a magnetic field is shown to induce a HSIT from a true zero-resistance superconducting state to a weakly insulating behavior. Determining the critical field, HC, we show that similar to the 2D behavior, the insulating-like state maintains a superconducting character, which is quenched at higher field, above which the magnetoresistance decreases to its fermionic normal state value.",2110.07251v3 2012-07-26,High pressure transport studies of the LiFeAs analogues CuFeTe2 and Fe2As,"We have synthesized two iron-pnictide/chalcogenide materials, CuFeTe2 and Fe2As, which share crystallographic features with known iron-based superconductors, and carried out high-pressure electrical resistivity measurements on these materials to pressures in excess of 30 GPa. Both compounds crystallize in the Cu2Sb-type crystal structure that is characteristic of LiFeAs (with CuFeTe2 exhibiting a disordered variant). At ambient pressure, CuFeTe2 is a semiconductor and has been suggested to exhibit a spin-density-wave transition, while Fe2As is a metallic antiferromagnet. The electrical resistivity of CuFeTe2, measured at 4 K, decreases by almost two orders of magnitude between ambient pressure and 2.4 GPa. At 34 GPa, the electrical resistivity decreases upon cooling the sample below 150 K, suggesting the proximity of the compound to a metal-insulator transition. Neither CuFeTe2 nor Fe2As superconduct above 1.1 K throughout the measured pressure range.",1207.6272v1 2012-10-12,Pressure Induced Superconductivity in Ba0.5Sr0.5Fe2As2,"High-pressure electrical resistance measurements have been performed on single crystal Ba0.5Sr0.5Fe2As2 platelets to pressures of 16 GPa and temperatures down to 10 K using designer diamond anvils under quasi-hydrostatic conditions with an insulating steatite pressure medium. The resistance measurements show evidence of pressure-induced superconductivity with an onset transition temperature at ~31 K and zero resistance at ~22 K for a pressure of 3.3 GPa. The transition temperature decreases gradually with increasing in pressure before completely disappearing for pressures above 12 GPa. The present results provide experimental evidence that a solid solution of two 122-type materials, e.g., Ba1-x.SrxFe2As2 (0 < x <1), can also exhibit superconductivity under high pressure",1210.3603v1 2012-12-03,Observation of Resistively Detected Hole Spin Resonance and Zero-field Pseudo-spin Splitting in Epitaxial Graphene,"Electronic carriers in graphene show a high carrier mobility at room temperature. Thus, this system is widely viewed as a potential future charge-based high-speed electronic-material to complement- or replace- silicon. At the same time, the spin properties of graphene have suggested improved capability for spin-based electronics or spintronics, and spin-based quantum computing. As a result, the detection, characterization, and transport of spin have become topics of interest in graphene. Here we report a microwave photo-excited transport study of monolayer and trilayer graphene that reveals an unexpectedly strong microwave-induced electrical-response and dual microwave-induced resonances in the dc-resistance. The results suggest the resistive detection of spin resonance, and provide a measurement of the g-factor, the spin relaxation time, and the sub-lattice degeneracy-splitting at zero-magnetic-field.",1212.0329v1 2013-04-09,Upper critical field of high quality single crystals of KFe$_2$As$_2$,"Measurements of temperature-dependent in-plane resistivity, $\rho(T)$, were used to determine the upper critical field and its anisotropy in high quality single crystals of stoichiometric iron arsenide superconductor KFe$_2$As$_2$. The crystals were characterized by residual resistivity ratio, $\rho(300K)/\rho(0)$ up to 3000 and resistive transition midpoint temperature, $T_c$=3.8 K, significantly higher than in previous studies on the same material. We find increased $H_{c2}(T)$ for both directions of the magnetic field, which scale with the increased $T_c$. This unusual linear $H_{c2}(T_c)$ scaling is not expected for orbital limiting mechanism of the upper critical field in clean materials.",1304.2689v1 2017-10-10,Thermal conductivity and electrical resistivity of solid iron at Earth's core conditions from first-principles,"We compute the thermal conductivity and electrical resistivity of solid hcp Fe to pressures and temperatures of Earth's core. We find significant contributions from electron-electron scattering, usually neglected at high temperatures in transition metals. Our calculations show a quasi-linear relation between electrical resistivity and temperature for hcp Fe at extreme high pressures. We obtain thermal and electrical conductivities that are consistent with experiments considering reasonable error. The predicted thermal conductivity is reduced from previous estimates that neglect electron-electron scattering. Our estimated thermal conductivity for the outer core is 77$\pm$10 W/m/K, and is consistent with a geodynamo driven by thermal convection.",1710.03564v6 2014-08-20,Carbon Memory Assessment,"The geometrical and performance scaling of silicon CMOS integrated circuit technology over the past 50 years has enabled many affordable new products for business and consumer applications. Recognizing that Flash is approaching its ultimate physical scaling limits within the next 10 years or so, the global electronics research community has begun an intense search for a new paradigm and technology for extending the functional scaling of memory technologies. Several promising nonvolatile memory concepts have emerged, based on different switching and retention mechanisms from those of Flash memory, e.g., STTRAM, RRAM, PCM and more recently, resistive memories based on carbon, which are the topic of this paper. This paper will introduce into the diverse field of carbon materials by recollecting some effects in carbon that can be used to produce a multiple time switchable, non-volatile unipolar resistive memory with potential high scalability down to atomic dimensions. Carbon-based memory is a non-volatile resistive memory, therefore, the same architectures, circuits, select transistor or diodes like in ReRAM or PCRAM can be considered as implementation. The big advantage of carbon memory might be the high temperature retention of 250 C, which makes it attractive for automotive and harsh conditions. This is a white paper for the ITRS meeting on emerging research devices (ERD) in Albuquerque, New Mexico, on August 25-26, 2014.",1408.4600v1 2003-11-06,"Violation of the Mott-Ioffe-Regel Limit: High-temperature Resistivity of Itinerant Magnets Srn+1RunO3n+1 (n=2,3,infinity) and CaRuO3","Srn+1RunO3n+1 represents a class of layered materials whose physical properties are a strong function of the number of Ru-O layers per unit cell, n. This series includes the p-wave superconductor Sr2RuO4 (n=1), enhanced paramagnetic Sr3Ru2O7 (n=2), nearly ferromagnetic Sr4Ru3O10 (n=3) and itinerant ferromagnetic SrRuO3 (n=infinity). In spite of a wide spectrum of physical phenomena, this series of materials along with paramagnetic CaRuO3 shares two major characteristics, namely, robust Fermi liquid behavior at low temperatures and anomalous transport behavior featured by linear temperature dependence of resistivity at high temperature where electron wavepackets are no longer clearly defined. There is no crossover separating such two fundamentally different states. In this paper, we report results of our study that systematically addresses anisotropy and temperature dependence of basal-plane and c-axis resistivity as a function of n for the entire Srn+1RunO3n+1 series and CaRuO3 and for a wide temperature range of 1.7 K TP) data were analyzed with Mott's small polaron hopping conduction mechanisms. PACS Codes: 73.50.Lw, 75.47.Gk, 75.47.Lx",0805.1663v1 2008-09-12,Two insulating phases in compressed Pr1-xCaxMnO3 thin films,"The temperature dependent resistivity of two Pr1-xCaxMnO3 (x=0.5 and 0.4) thin films grown on LaAlO3 has been studied as a function of hydrostatic pressure (up to 2.5 GPa) and magnetic field (up to 9T). Both samples show a monotonic decrease in the resistivity with an increase in pressure, corresponding to a change of -35% at 2.5 GPa. No pressure induced metal-to-insulator transition was observed in the temperature-dependent resistivity. The non-trivial interaction between high pressure and magnetic field reveals that the effect of pressure cannot be simply rescaled to that of a specific field, as has been reported for the corresponding bulk material. We propose an interpretation of the data based on phase separation, where two different insulating phases coexist: the charge ordered phase, which is sensitive to both magnetic field and pressure, and a second insulating phase that can be tuned by magnetic field. Such a result demonstrates that phase separation can be manipulated in thin films by independent application of magnetic field and/or external pressure.",0809.2184v1 2008-10-28,Electrical properties of boron-doped MWNTs synthesized by hot-filament chemical vapor deposition,"We have synthesized a large amount of boron-doped multiwalled carbon nanotubes (MWNTs) by hot-filament chemical vapor deposition. The synthesis was carried out in a flask using a methanol solution of boric acid as a source material. The scanning electron microscopy, transmission electron microscopy, and micro-Raman spectroscopy were performed to evaluate the structural properties of the obtained MWNTs. In order to evaluate the electrical properties, temperature dependence of resistivity was measured in an individual MWNTs with four metal electrodes. The Ramman shifts suggest carrier injection into the boron-doped MWNTs, but the resistivity of the MWNTs was high and increased strongly with decreasing temperature. Defects induced by the plasma may cause this enhanced resistivity.",0810.4971v1 2011-06-15,An Analytical Approach for Memristive Nanoarchitectures,"As conventional memory technologies are challenged by their technological physical limits, emerging technologies driven by novel materials are becoming an attractive option for future memory architectures. Among these technologies, Resistive Memories (ReRAM) created new possibilities because of their nano-features and unique $I$-$V$ characteristics. One particular problem that limits the maximum array size is interference from neighboring cells due to sneak-path currents. A possible device level solution to address this issue is to implement a memory array using complementary resistive switches (CRS). Although the storage mechanism for a CRS is fundamentally different from what has been reported for memristors (low and high resistances), a CRS is simply formed by two series bipolar memristors with opposing polarities. In this paper our intention is to introduce modeling principles that have been previously verified through measurements and extend the simulation principles based on memristors to CRS devices and hence provide an analytical approach to the design of a CRS array. The presented approach creates the necessary design methodology platform that will assist designers in implementation of CRS devices in future systems.",1106.2927v2 2013-02-05,Graphene-Ferroelectric Hybrid Structure for Flexible Transparent Electrodes,"Graphene has exceptional optical, mechanical and electrical properties, making it an emerging material for novel optoelectronics, photonics and for flexible transparent electrode applications. However, the relatively high sheet resistance of graphene is a major constrain for many of these applications. Here we propose a new approach to achieve low sheet resistance in large-scale CVD monolayer graphene using non-volatile ferroelectric polymer gating. In this hybrid structure, large-scale graphene is heavily doped up to 3{\times}1013 cm-2 by non-volatile ferroelectric dipoles, yielding a low sheet resistance of 120 {\Omega}{\Box} at ambient conditions. The graphene-ferroelectric transparent conductors (GFeTCs) exhibit more than 95% transmittance from the visible to the near infrared range owing to the highly transparent nature of the ferroelectric polymer. Together with its excellent mechanical flexibility, chemical inertness and the simple fabrication process of ferroelectric polymers, the proposed GFeTCs represent a new route towards large-scale graphene based transparent electrodes and optoelectronics.",1302.0993v1 2013-03-11,"Crystals, magnetic and electronic properties of a new ThCr2Si2-type BaMn2Bi2 and K-doped compositions","This is a report on the new 122 ternary transition-metal pnictide of BaMn2Bi2, which is crystallized from bismuth flux. BaMn2Bi2 adopts ThCr2Si2-type structure (I4/mmm) with a = 4.4902(3) {\AA} and c = 14.687(1) {\AA}; it is antiferromagnetic with anisotropic magnetic susceptibility and semiconducting with a band gap of Eg = 6 meV. Heat capacity result confirms the insulating ground state in BaMn2Bi2 with the electronic residual Sommerfeld coefficient of {\gamma} ~ 0. The high temperature magnetization results show that magnetic ordering temperature is TN ~ 400 K. Hole-doping in BaMn2Bi2 via potassium in Ba1-xKxMn2Bi2 results in metallic behavior for x = 0.10(1), 0.32(1) and 0.36(1). With K-doping, more magnetically anisotropic behavior is observed. Although there is a downturn in electrical resistivity and low-field magnetization data below 4 K in > 30%-doped crystals, there is no sign of zero resistance or diamagnetism. This manuscript is a report on new materials of BaMn2Bi2 and Ba1-xKxMn2Bi2 (0 < x < 0.4). Results from powder X-ray diffraction, anisotropic temperature- and field-dependent magnetization, temperature-and field-dependent electrical resistivity, and heat capacity are presented.",1303.2695v2 2015-02-09,Surface-state-dominated transport in crystals of the topological crystalline insulator In-doped Pb$_{1-x}$Sn$_x$Te,"Three-dimensional topological insulators and topological crystalline insulators represent new quantum states of matter, which are predicted to have insulating bulk states and spin-momentum-locked gapless surface states. Experimentally, it has proven difficult to achieve the high bulk resistivity that would allow surface states to dominate the transport properties over a substantial temperature range. Here we report a series of indium-doped Pb$_{1-x}$Sn$_x$Te compounds that manifest huge bulk resistivities together with strong evidence of topological surface states, based on thickness-dependent transport studies and magnetoresistance measurements. For these bulk-insulating materials, the surface states determine the resistivity for temperatures approaching 30 K.",1502.02696v1 2016-04-20,Magnetoresistance and Shubnikov-de Hass oscillation in YSb,"YSb crystals are grown and the transport properties under magnetic field are measured. The resistivity exhibits metallic behavior under zero magnetic field and the low temperature resistivity shows a clear upturn once a moderate magnetic field is applied. The upturn is greatly enhanced by increasing magnetic field, finally resulting in a metal-to-insulator-like transition. With temperature further decreased, a resistivity plateau emerges after the insulator-like regime. At low temperature (2.5 K) and high field (14 T), the transverse magnetoresistance (MR) is quite large (3.47 $\times 10^4\%$ ). In addition, Shubnikov-de Haas (SdH) oscillation has also been observed in YSb. Periodic behavior of the oscillation amplitude reveals the related information about Fermi surface and two major oscillation frequencies can be obtained from the FFT spectra of the oscillations. The trivial Berry phase extracted from SdH oscillation, band structure revealed by angle-resolved photoemission spectroscopy (ARPES) and first-principles calculations demonstrate that YSb is a topologically trivial material.",1604.05912v2 2016-04-06,Structural characterization of APPJ treated Bismaleimide coatings and heat treated Titania-BMI,"Bismaleimide (BMI) are thermosetting polymers mainly used in aerospace applications having properties of dimensional stability, low shrinkage, chemical resistance, fire resistance, good mechanical properties and high resistance against various solvents, acids, and water. BMI is commercially available as Homide 250. BMI coating has also been used for the corrosion protection. Metallization (AL) of BMI using vacuum evaporation was done which serves the purpose of prevention of space charge accumulation in aircraft bodies. Addition of inorganic materials like metal oxides can influence the properties of the polymer as an inorganic-organic composite. The organic-ionorganic composites have wide applications in electronics, optics, chemistry and medicine. Titanium dioxide (TiO2, Titania) has a wide range of applications starting from photocatalysis, dye-sensitized solar cells to optical coatings and electronics. A BMI-TiO2 composite was prepared by chemical route. Atmospheric Plasma Jet (APPJ) using Helium gas was also treated on BMI. XRD and FTIR studies of the composite system prepared at different temperatures showed its crystalline and structural configuration.",1604.07297v1 2016-06-27,Structural and electrical properties of Sn substituted double sintering derived Ni-Zn ferrite,"The Sn substituted Ni-Zn ferrites were synthesized by the standard double sintering technique using nano powders of nickel oxide (NiO), zinc oxide (ZnO), iron oxide (Fe2O3) and tin oxide (SnO2). The structural and electrical properties have been investigated by the X-ray diffraction, scanning electron microscopy, DC resistivity and dielectric measurements. Extra intermediate phase has been detected along with the inverse cubic spinel phase of Ni-Zn ferrite. Enhancement of grain size is observed in Sn substituted Ni-Zn ferrites. DC resistivity as a function of temperature has been investigated by two probe method. The DC resistivity was found to decrease whereas the dielectric constants increase with increasing Sn content in Ni-Zn ferrites. The dielectric constant of the as prepared samples is high enough to use these materials in miniaturized memory devices based capacitive components or energy storage principles.",1606.08118v1 2017-02-18,Scaling limits of graphene nanoelectrodes,"Graphene is an ideal material for fabricating atomically thin nanometre spaced electrodes. Recently, carbon-based nanoelectrodes have been employed to create single-molecule transistors and phase change memory devices. In spite of the significant recent interest in their use in a range of nanoscale devices from phase change memories to molecular electronics, the operating and scaling limits of these electrodes are completely unknown. In this paper, we report on our observations of consistent voltage driven resistance switching in sub-5 nm graphene nanogaps. We find that we are able to reversibly cycle between a low and a high resistance state using feedback-controlled voltage ramps.We attribute this unexplained switching in the gap to the formation and breakdown of carbon filaments.By increasing the gap, we find that such intrinsic resistance switching of graphene nanogaps imposes a scaling limit of 10 nm (approx.) on the gap-size for devices with operating voltages of 1 to 2 volts.",1702.05668v1 2019-09-23,Nanoscale ballistic diodes made of polar materials for amplification and generation of radiation in 10 THz-range,"We investigate ultra-high frequency electrical properties of nanoscale $n^+$-$i$-$n^+$ diodes made of polar semiconductors. The calculations show that the coupling between optical vibrations of the lattice and the ballistic electrons strongly modifies and enhances the time-of-flight effects giving rise to narrow resonances of the diode impedance in the reststrahlen frequency range. Particularly, negative dynamic resistance is induced in close proximity to the optical phonon frequency. The resonant effects in the dynamic resistance of nanoscale GaAs and InP diodes are studied in detail. The obtained magnitudes of the negative dynamic resistance effect indicate that the nanoscale diodes are capable of generating electromagnetic radiation in far-infrared spectral range under electric pumping.",1909.10185v1 2019-12-20,Electron-phonon interaction and zero-field charge carrier transport in the nodal-line semimetal ZrSiS,"We study electron-phonon interaction and related transport properties of nodal-line semimetal ZrSiS using first-principles calculations. We find that ZrSiS is characterized by a weak electron-phonon coupling on the order of 0.1, which is almost energy independent. The main contribution to the electron-phonon coupling originates from long-wavelength optical phonons, causing no significant renormalization of the electron spectral function. At the charge neutrality point, we find that electrons and holes provide a comparable contribution to the scattering rate. The phonon-limited resistivity calculated within the Boltzmann transport theory is found to be strongly direction-dependent with the ratio between out-of-plane and in-plane directions being $\rho_{zz}/\rho_{xx}\sim 7.5$, mainly determined by the anisotropy of carrier velocities. We estimate zero-field resistivity to be $\rho_{xx}\approx12$ $\mu\Omega$ cm at 300 K, which is in good agreement with experimental data. Relatively small resistivity in ZrSiS can be attributed to a combination of weak electron-phonon coupling and high carrier velocities.",1912.09832v2 2015-04-06,Gate-tunable Memristive Phenonmena Mediated by Grain Boundaries in Single Layer MoS2,"Continued progress in high speed computing depends on breakthroughs in both materials synthesis and device architectures. The performance of logic and memory can be enhanced significantly by introducing a memristor, a two terminal device with internal resistance that depends on the history of the external bias voltage. State of the art memristors, based on metal insulator metal (MIM) structures with insulating oxides, such as TiO2, are limited by a lack of control over the filament formation and external control of the switching voltage. Here, we report a class of memristors based on grain boundaries (GBs) in single-layer MoS2 devices. Specifically, the resistance of GBs emerging from contacts can be easily and repeatedly modulated, with switching ratios up to 1000 and a dynamic negative differential resistance (NDR). Furthermore, the atomically thin nature of MoS2 enables tuning of the set voltage by a third gate terminal in a field-effect geometry, which provides new functionality that is not observed in other known memristive devices.",1504.01416v1 2020-12-09,"Potassium-Doped Para-Terphenyl: Structure, Electrical Transport Properties and Possible Signatures of a Superconducting Transition","Preliminary evidence for the occurrence of high-Tc superconductivity in alkali-doped organic materials, such as potassium-doped p-terphenyl (KPT), were recently obtained by magnetic susceptibility measurements and by the opening of a large superconducting gap as measured by ARPES and STM techniques. In this work, KPT samples have been synthesized by a chemical method and characterized by low-temperature Raman scattering and resistivity measurements. Here, we report the occurrence of a resistivity drop of more than 4 orders of magnitude at low temperatures in KPT samples in the form of compressed powder. This fact was interpreted as a possible sign of a broad superconducting transition taking place below 90 K in granular KPT. The granular nature of the KPT system appears to be also related to the 20 K broadening of the resistivity drop around the critical temperature.",2012.04899v1 2020-12-23,Direct observation of the electrically triggered Insulator-Metal transition in V3O5 far below the transition temperature,"Resistive switching is one of the key phenomena for applications such as nonvolatile memories or neuromorphic computing. V3O5, a compound of the vanadium oxide Magn\'eli series, is one of the rare materials to exhibit an insulator-metal transition (IMT) above room temperature (Tc ~ 415 K). Here we demonstrate both static dc resistive switching (RS) and fast oscillatory spiking regimes in V3O5 devices at room temperature (120 K below the phase transition temperature) by applying an electric field. We use operando optical imaging to track a reflectivity change during the RS and find that a percolating high temperature metallic phase filament is formed. This demonstrates that the electrically induced RS triggers the phase transition. Furthermore, we optically capture the spiking oscillations that we link to the negative differential resistance regime and find the filament forms and dissolves via a periodic spatio-temporal instability that we describe by numerical simulations.",2012.13009v1 2021-02-10,Current-limiting amplifier for high speed measurement of resistive switching data,"Resistive switching devices, important for emerging memory and neuromorphic applications, face significant challenges related to control of delicate filamentary states in the oxide material. As a device switches, its rapid conductivity change is involved in a positive feedback process that would lead to runaway destruction of the cell without current, voltage, or energy limitation. Typically, cells are directly patterned on MOS transistors to limit the current, but this approach is very restrictive as the necessary integration limits the materials available as well as the fabrication cycle time. In this article we propose an external circuit to cycle resistive memory cells, capturing the full transfer curves while driving the cells in such a way to suppress runaway transitions. Using this circuit, we demonstrate the acquisition of $10^5$ I-V loops per second without the use of on-wafer current limiting transistors. This setup brings voltage sweeping measurements to a relevant timescale for applications, and enables many new experimental possibilities for device evaluation in a statistical context.",2102.05770v1 2021-04-13,Negative Differential Resistance in Carbon-Based Nanostructures,"Nonlinear electrical properties, such as negative differential resistance (NDR), are essential in numerous electrical circuits, including memristors. Several physical origins have been proposed to lead to the NDR phenomena in semiconductor devices in the last more than half a century. Here, we report NDR behavior formation in randomly oriented graphene-like nanostructures up to 37 K and high on-current density up to 10^5 A/cm^2. Our modeling of the current-voltage characteristics, including the self-heating effects, suggests that strong temperature dependence of the low-bias resistance is responsible for the nonlinear electrical behavior. Our findings open opportunities for the practical realization of the on-demand NDR behavior in nanostructures of 2D and 3D material-based devices via heat management in the conducting films and the underlying substrates.",2104.06337v2 2021-05-17,Enhancement of the superconductivity and quantum metallic state in the thin film of superconducting Kagome metal KV$_3$Sb$_5$,"Recently V-based Kagome metal attracted intense attention due to the emergence of superconductivity in the low temperature. Here we report the fabrication and physical investigations of the high quality single-crystalline thin films of the Kagome metal KV$_3$Sb$_5$. For the sample with the thickness of about 15 nm, the temperature dependent resistance reveals a Berezinskii-Kosterlitz-Thouless (BKT) type behavior, indicating the presence of two-dimensional superconductivity. Compared with the bulk sample, the onset transition temperature $T^{onset}_{c}$ and the out-of-plane upper critical field $H_{c2}$ are enhanced by 15\% and more than 10 times respectively. Moreover, the zero-resistance state is destroyed by a magnetic field as low as 50 Oe. Meanwhile, the temperature-independent resistance is observed in a wide field region, which is the hallmark of quantum metallic state. Our results provide evidences for the existence of unconventional superconductivity in this material.",2105.07732v1 2021-06-28,Superconductivity in an extreme strange metal,"Some of the highest-transition-temperature superconductors across various materials classes exhibit linear-in-temperature `strange metal' or `Planckian' electrical resistivities in their normal state. It is thus believed by many that this behavior holds the key to unlock the secrets of high-temperature superconductivity. However, these materials typically display complex phase diagrams governed by various competing energy scales, making an unambiguous identification of the physics at play difficult. Here we use electrical resistivity measurements into the micro-Kelvin regime to discover superconductivity condensing out of an extreme strange metal state -- with linear resistivity over 3.5 orders of magnitude in temperature. We propose that the Cooper pairing is mediated by the modes associated with a recently evidenced dynamical charge localization-delocalization transition, a mechanism that may well be pertinent also in other strange metal superconductors.",2106.14849v2 2022-01-28,"Factors that control stability, variability, and reliability issues of endurance cycle in ReRAM devices: a phase field study","The morphological evolution of the conducting filament (CF) predominantly controls the electric response of the resistive random access memory (ReRAM) devices. However, the parameters -- in terms of the material and the processing -- which control the growth of such CF are plenty. Extending the phase field technique for ReRAM systems presented by Roy and Cha [J. Appl. Phys. 128, 205102 (2020)], we could successfully model the complete SET (low resistance state) and RESET (high resistance state) sates due to the application of sweeping voltage. The key parameters that influence the stability of the multi-cycle \emph{I-V} response or the endurance behavior are identified. The computational findings of the presented model ReRAM system are practical in correlating the multi-parametric influence with the stability, variability, and reliability of the endurance cycle that affect the device performance and also lead to the device failure. We believe that our computational approach of connecting the morphological changes of the CF with the electrical response, has the potential to further understand and optimize the performance of the ReRAM devices.",2201.12304v2 2022-07-03,An Atomistic Modelling Framework for Valence Change Memory Cells,"We present a framework dedicated to modelling the resistive switching operation of Valence Change Memory (VCM) cells. The method combines an atomistic description of the device structure, a Kinetic Monte Carlo (KMC) model for the creation and diffusion of oxygen vacancies in the central oxide under an external field, and an ab-initio quantum transport method to calculate electrical current and conductance. As such, it reproduces a realistically stochastic device operation and its impact on the resulting conductance. We demonstrate this framework by simulating a switching cycle for a TiN/HfO$_2$/TiN VCM cell, and see a clear current hysteresis between high/low resistance states, with a conductance ratio of one order of magnitude. Additionally, we observe that the changes in conductance originate from the creation and recombination of vacancies near the active electrode, effectively modulating a tunnelling gap for the current. This framework can be used to further investigate the mechanisms behind resistive switching at an atomistic scale and optimize VCM material stacks and geometries.",2207.01095v1 2023-06-16,Piezo-resistive pressure sensor based on CVD-grown ZnO nanowires on Polyethylene Tetrathalate substrate,"Recent developments in the domain of electronic materials and devices have attracted the interest of researchers toward flexible and printable electronic components like organic transistors, printable electrodes and sensors. Zinc Oxide (ZnO) nanowires (NWs) possess a number of excellent properties like high mobility, large exciton binding energy and the direct-band gap in addition to large piezoelectric coefficients. Here, we report on flexible piezo-resistive sensor based on Indium tin oxide (ITO)-coated Polyethylene tetrathalate (PET) substrate. The device shows sensitivity in terms of change in resistance from 100 {\Omega} to 2.4 K{\Omega} at an applied potential of 5V upon bending from flat to 95 degrees. The 1-D nanowire flexible device in its flat state shows saturated output current. We observed ten folds enhanced variation as compared to previous reports. Improved sensitivity was observed in our experiments due to fewer defects in CVD-grown NWs as compared to others where hydrothermally grown nanowires were used. The methodology of device fabrication reported here requires less time and enables efficient devices for the realization of flexible and wearable technology.",2307.13805v1 2023-10-22,Microstructure evolution and characteristics of laser-clad lightweight refractory NbxMo$_{0.5}$Ti$_{1.5}$Ta$_{0.2}$Cr high-entropy alloy,"Lightweight refractory high-entropy alloy coatings (RHEAcs) of NbxMo$_{0.5}$Ti$_{1.5}$Ta$_{0.2}$Cr (where $x=$ 1, 1.3, 1.5, and 2) were fabricated on the surface of 316L stainless steel using laser cladding (LC) technology. A comprehensive study was conducted to elucidate the effect of Nb content on the microstructure, microhardness and wear resistance of NbxMo$_{0.5}$Ti$_{1.5}$Ta$_{0.2}$Cr RHEAcs before and after annealing at 900 for 10 h. The results show that the grains are gradually refined with the increase of Nb content. The coating consists mainly of a body-centered cubic (BCC) solid solution, C15-Laves phase, and a small amount of hexagonal close-packed (HCP) solid solution containing Ti. The microhardness of RHEAcs is significantly higher compared to the base material. Notably, at Nb1.3, due to the influence of lattice dislocations, the microhardness reaches a peak of 1066.5 HV, which is about 7.11 times higher than that of the base material. On the contrary, at Nb$_2$, the microhardness is at its lowest point, averaging 709.31 HV, but 4.72 times that of the base material. After annealing, an increase in microhardness is observed at all Nb concentrations, up to 31.2% at Nb$_2$. Before annealing, the wear resistance of RHEAcs was slightly better than that of 316L stainless steel at different Nb contents. However, after annealing, the coefficient of friction (COF) and wear rate of the coatings are lower than those of annealed 316L stainless steel, highlighting their excellent wear resistance. It is noteworthy that the loss of wear properties after annealing at Nb1 is at a minimum, obtaining the most balanced wear resistance before and after annealing. The enhanced wear resistance after annealing can be attributed to the presence of ultra-fine grain oxide friction layers, mainly composed of TiO2 and Ta2O5 . The main mode of wear is oxidative wear, with a small amount of wear from abrasive wear.",2310.14223v1 2019-08-16,Scaling Analysis of Anomalous Hall Resistivity in the Co$_{2}$TiAl Heusler Alloy,"A comprehensive magnetotransport study including resistivity ($\rho_{xx}$) at various fields, isothermal magnetoresistance and Hall resistivity ($\rho_{xy}$) has been carried out at different temperatures on the Co$_{2}$TiAl Heusler alloy. Co$_{2}$TiAl alloy shows a paramagnetic (PM) to ferromagnetic (FM) transition below the curie temperature (T$_{C}$) $\sim$ 125 K. In the FM region, resistivity and magnetoresistance reveals a spin flip electron-magnon scattering and the Hall resistivity unveils the anomalous Hall resistivity ($\rho_{xy}^{AH}$). Scaling of anomalous Hall resistivity with resistivity establishes the extrinsic scattering process responsible for the anomalous hall resistivity; however Skew scattering is the dominant mechanism compared to the side-jump contribution. A one to one correspondence between magnetoresistance and side-jump contribution to anomalous Hall resistivity verifies the electron-magnon scattering being the source of side-jump contribution to the anomalous hall resistivity.",1908.05974v1 2009-08-20,"Magnetism, Superconductivity and Stoichiometry in Single Crystals of Fe1+y(Te1-xSx)z","We report synthesis of high quality Fe1+y(Te1-xSx)z single crystals and a comprehensive study of structural, magnetic and transport properties. There is high sensitivity to material stoichiometry which includes vacancies on the Te(S) site. Our results reveal competition and coexistence of magnetic order and percolative superconductivity for x >= 0.03, while zero resistivity is acheived for x >= 0.1.",0908.3011v1 2020-11-20,"Phonons, electrons and thermal transport in Planckian high T$_c$ materials","The room temperature thermal diffusivity of high T$_c$ materials is dominated by phonons. This allows the scattering of phonons by electrons to be discerned. We argue that the measured strength of this scattering suggests a converse Planckian scattering of electrons by phonons across the room temperature phase diagram of these materials. Consistent with this conclusion, the temperature derivative of the resistivity of strongly overdoped cuprates is noted to show a kink at a little below 200 K that we argue should be understood as the onset of a high temperature Planckian $T$-linear scattering of electrons by classical phonons. This kink continuously disappears towards optimal doping, even while strong scattering of phonons by electrons remains visible in the thermal diffusivity, sharpening the long-standing puzzle of the lack of a feature in the $T$-linear resistivity at optimal doping associated to onset of phonon scattering.",2011.10466v2 2017-08-10,Zero resistance from one atmosphere to the pressure of earth's outer core in a superconducting high entropy alloy,"We report the observation of extraordinarily robust zero-resistance superconductivity in the pressurized (TaNb)0.67(HfZrTi)0.33 high entropy alloy - a new kind of material with a body-centered cubic crystal structure made from five randomly distributed transition metal elements. The transition to superconductivity (TC) increases from an initial temperature of 7.7 K at ambient pressure to 10 K at ~ 60 GPa, and then slowly decreases to 9 K by 190.6 GPa, a pressure that falls within that of the outer core of the earth. We infer that the continuous existence of the zero-resistance superconductivity from one atmosphere up to such a high pressure requires a special combination of electronic and mechanical characteristics. This high entropy alloy superconductor thus may have a bright future for applications under extreme conditions, and also poses a challenge for understanding the underlying quantum physics.",1708.03146v2 2020-05-16,Electric-field induced strange metal states and possible high-temperature superconductivity in hydrogenated graphitic fibers,"In this work, we have studied the effects from increasing the strength of the applied electric field on the charge transport of hydrogenated graphitic fibers. Resistivity measurements were carried out for direct currents in the nA - mA range and for temperatures from 1.9 K to 300 K. The high-temperature non-ohmic voltage-current dependence is well described by the nonlinear random resistor network model applied to systems that are disordered at all scales. The temperature-dependent resistivity shows linear, step-like transitions from insulating to metallic states as well as plateau features. As more current is being sourced, the fiber becomes more conductive and thus the current density goes up. The most interesting features is observed in high electric fields. As the fiber is cooled, the resistivity first decreases linearly with the temperature and then enters a plateau region at a temperature T ? 260 ? 280 K that is field-independent. These observations on a system made out of carbon, hydrogen, nitrogen, and oxygen atoms suggest possible electric-field induced superconductivity with a high critical temperature that was predicted from studying the role of chirality on the origin of life [1].",2005.07885v1 2021-09-28,Development of high-rate capable and ultra-low mass Resistive Plate Chamber with Diamond-Like Carbon,"A new type of resistive plate chamber (RPC) is under development using thin-film resistive electrodes based on diamond-like carbon (DLC). Planned to be put on the path of high-intensity low-momentum muon beam of the MEG II experiment, this detector is required to be high-rate capable and ultra-low mass. Using a prototype detector with 2 cm $\times$ 2 cm size and 0.1 % $X_0$ material budget, performance studies were conducted for MIP detection efficiency, timing resolution and high rate capability in low-momentum muon beam. In this paper, the measured performance is presented including the result with low-momentum muon beam at rate up to 1 $\mathrm{MHz/cm^2}$. Based on the result, the expected performance of the full-scale detector in the MEG~II experiment is also discussed.",2109.13525v1 2014-02-06,High-performance ferroelectric memory based on fully patterned tunnel junctions,"In tunnel junctions with ferroelectric barriers, switching the polarization direction modifies the electrostatic potential profile and the associated average tunnel barrier height. This results in strong changes of the tunnel transmission and associated resistance. The information readout in ferroelectric tunnel junctions (FTJs) is thus resistive and non-destructive, which is an advantage compared to the case of conventional ferroelectric memories (FeRAMs). Initially, endurance limitation (i.e. fatigue) was the main factor hampering the industrialization of FeRAMs. Systematic investigations of switching dynamics for various ferroelectric and electrode materials have resolved this issue, with endurance now reaching $10^{14}$ cycles. Here we investigate data retention and endurance in fully patterned submicron Co/BiFeO$_3$/Ca$_{0.96}$Ce$_{0.04}$MnO$_3$ FTJs. We report good reproducibility with high resistance contrasts and extend the maximum reported endurance of FTJs by three orders of magnitude ($4\times10^6$ cycles). Our results indicate that here fatigue is not limited by a decrease of the polarization or an increase of the leakage but rather by domain wall pinning. We propose directions to access extreme and intermediate resistance states more reliably and further strengthen the potential of FTJs for non-volatile memory applications.",1402.1289v1 2021-07-02,Topological surface conduction in Kondo insulator YbB$_{12}$,"Kondo insulators have recently aroused great interest because they are promising materials that host a topological insulator state caused by the strong electron interactions. Moreover, recent observations of the quantum oscillations in the insulating state of Kondo insulators have come as a great surprise. Here, to investigate the surface electronic state of a prototype Kondo insulator YbB$_{12}$, we measured transport properties of single crystals and microstructures. In all samples, the temperature dependence of the electrical resistivity is insulating at high temperatures and the resistivity exhibits a plateau at low temperatures. The magnitude of the plateau value decreases with reducing sample thickness, which is quantitatively consistent with the surface electronic conduction in the bulk insulating YbB$_{12}$. Moreover, the magnetoresistance of the microstructures exhibits a weak-antilocalization effect at low field. These results are consistent with the presence of topologically protected surface state, suggesting that YbB$_{12}$ is a candidate material of the topological Kondo insulator. The high field resistivity measurements up to $\mu_0H$ = 50 T of the microstructures provide supporting evidence that the quantum oscillations of the resistivity in YbB$_{12}$ occurs in the insulating bulk.",2107.00912v2 2021-07-22,Quantum oscillations in 2D insulators induced by graphite gates,"We demonstrate a mechanism for magnetoresistance oscillations in insulating states of two-dimensional (2D) materials arising from the interaction of the 2D layer and proximal graphite gates. We study a series of devices based on different two-dimensional systems, including mono- and bilayer Td-WTe2, angle-aligned MoTe2/WSe2 heterobilayers and Bernal-stacked bilayer graphene, which all share a similar graphite-gated geometry. We find that the resistivity of the 2D system generically shows quantum oscillations as a function of magnetic field corresponding to a high-density Fermi surface when they are tuned near an insulating state, in contravention of na\""ive band theory. Simultaneous measurement of the resistivity of the graphite gates show that these oscillations are precisely correlated with quantum oscillations in the resistivity of the graphite gates themselves. Further supporting this connection, the oscillations are quenched when the graphite gate is replaced by TaSe2, a high-density metal that does not show quantum oscillations. The observed phenomenon arises from the oscillatory behavior of graphite density of states, which modulates the device capacitance and, as a consequence, the carrier density in the sample layer even when a constant electrochemical potential is maintained between the sample and the gate electrode. Oscillations are most pronounced near insulating states where the resistivity is strongly density dependent. Our study suggests a unified mechanism for quantum oscillations in graphite-gated 2D insulators based on sample-gate coupling.",2107.10430v2 2014-11-10,Low carrier concentration crystals of the topological insulator Bi$_{2-x}$Sb$_{x}$Te$_{3-y}$Se$_{y}$: a magnetotransport study,"In 3D topological insulators achieving a genuine bulk-insulating state is an important research topic. Recently, the material system (Bi,Sb)$_{2}$(Te,Se)$_{3}$ (BSTS) has been proposed as a topological insulator with high resistivity and a low carrier concentration (Ren \textit{et al.} \cite{Ren2011}). Here we present a study to further refine the bulk-insulating properties of BSTS. We have synthesized Bi$_{2-x}$Sb${_x}$Te$_{3-y}$Se$_{y}$ single crystals with compositions around $x = 0.5$ and $y = 1.3$. Resistance and Hall effect measurements show high resistivity and record low bulk carrier density for the composition Bi$_{1.46}$Sb$_{0.54}$Te$_{1.7}$Se$_{1.3}$. The analysis of the resistance measured for crystals with different thicknesses within a parallel resistor model shows that the surface contribution to the electrical transport amounts to 97% when the sample thickness is reduced to $1 \mu$m. The magnetoconductance of exfoliated BSTS nanoflakes shows 2D weak antilocalization with $\alpha \simeq -1$ as expected for transport dominated by topological surface states.",1411.2479v2 2022-05-20,Resistivity and Thermal Conductivity of an Organic Insulator beta'-EtMe3Sb[Pd(dmit)2]2,"A finite residual linear term in the thermal conductivity at zero temperature in insulating magnets indicates the presence of gapless excitations of itinerant quasiparticles, which has been observed in some candidate materials of quantum spin liquids (QSLs). In the organic triangular insulator beta'-EtMe3Sb[Pd(dmit)2]2, a QSL candidate material, the low-temperature thermal conductivity depends on the cooling process and the finite residual term is observed only in samples with large thermal conductivity. Moreover, the cooling rate dependence is largely sample dependent. Here we find that, while the low-temperature thermal conductivity significantly depends on the cooling rate, the high-temperature resistivity is almost perfectly independent of the cooling rate. These results indicate that in the samples with the finite residual term, the mean free path of the quasiparticles that carry the heat at low temperatures is governed by disorders, whose characteristic length scale of the distribution is much longer than the electron mean free path that determines the high-temperature resistivity. This explains why recent X-ray diffraction and nuclear magnetic resonance measurements show no cooling rate dependence. Naturally, these measurements are unsuitable for detecting disorders of the length scale relevant for the thermal conductivity, just as they cannot determine the residual resistivity of metals. Present results indicate that very careful experiments are needed when discussing itinerant spin excitations in beta'-EtMe3Sb[Pd(dmit)2]2.",2205.10039v1 2022-09-17,Superfunctional high-entropy alloys and ceramics by severe plastic deformation,"High-entropy alloys and ceramics containing at least five principal elements have recently received high attention for various mechanical and functional applications. The application of severe plastic deformation (SPD), particularly the high-pressure torsion (HPT) method, combined with the CALPHAD and first-principles calculations resulted in the development of numerous superfunctional high-entropy materials with superior properties compared to the normal functions of engineering materials. This article reviews the recent advances in the application of SPD to developing superfunctional high-entropy materials. These superfunctional properties include (i) ultrahigh hardness levels comparable to the hardness of ceramics in high-entropy alloys, (ii) high yield strength and good hydrogen embrittlement resistance in high-entropy alloys; (iii) high strength, low elastic modulus, and high biocompatibility in high-entropy alloys, (iv) fast and reversible hydrogen storage in high-entropy hydrides, (v) photovoltaic performance and photocurrent generation on high-entropy semiconductors, (vi) photocatalytic oxygen and hydrogen production from water splitting on high-entropy oxides and oxynitrides, and (vii) CO2 photoreduction on high-entropy ceramics. These findings introduce SPD as not only a processing tool to improve the properties of existing high-entropy materials but also as a synthesis tool to produce novel high-entropy materials with superior properties compared with conventional engineering materials.",2209.08291v3 2016-06-10,Short channel effects in graphene-based field effect transistors targeting radio-frequency applications,"Channel length scaling in graphene field effect transistors (GFETs) is key in the pursuit of higher performance in radio frequency electronics for both rigid and flexible substrates. Although two-dimensional (2D) materials provide a superior immunity to Short Channel Effects (SCEs) than bulk materials, they could dominate in scaled GFETs. In this work, we have developed a model that calculates electron and hole transport along the graphene channel in a drift-diffusion basis, while considering the 2D electrostatics. Our model obtains the self-consistent solution of the 2D Poisson's equation coupled to the current continuity equation, the latter embedding an appropriate model for drift velocity saturation. We have studied the role played by the electrostatics and the velocity saturation in GFETs with short channel lengths L. Severe scaling results in a high degradation of GFET output conductance. The extrinsic cutoff frequency follows a 1/L^n scaling trend, where the index n fulfills n < 2. The case n = 2 corresponds to long-channel GFETs with low source/drain series resistance, that is, devices where the channel resistance is controlling the drain current. For high series resistance, n decreases down to n= 1, and it degrades to values of n < 1 because of the SCEs, especially at high drain bias. The model predicts high maximum oscillation frequencies above 1 THz for channel lengths below 100 nm, but, in order to obtain these frequencies, it is very important to minimize the gate series resistance. The model shows very good agreement with experimental current voltage curves obtained from short channel GFETs and also reproduces negative differential resistance, which is due to a reduction of diffusion current.",1606.03264v2 2007-01-29,Long-term Correlations and 1/f^alpha Noise in the Steady States of Multi-Species Resistor Networks,"We introduce a multi-species network model which describes the resistance fluctuations of a resistor in a non-equilibrium stationary state. More precisely, a thin resistor characterized by a 1/f^alpha resistance noise is described as a two-dimensional network made by different species of elementary resistors. The resistor species are distinguished by their resistances and by their energies associated with thermally activated processes of breaking and recovery. Depending on the external conditions, stationary states of the network can arise as a result of the competition between these processes. The properties of the network are studied as a function of the temperature by Monte Carlo simulations carried out in the temperature range 300 \div 800 K. At low temperatures, the resistance fluctuations display long-term correlations expressed by a power-law behavior of the auto-correlation function and by a value approx 1 of the alpha-exponent of the spectral density. On the contrary, at high temperatures the resistance fluctuations exhibit a finite and progressively smaller correlation time associated with a non-exponential decay of correlations and with a value of the alpha-exponent smaller than one. This temperature dependence of the alpha coefficient reproduces qualitatively well the experimental findings.",0701712v1 2008-06-26,Different resistivity response to spin density wave and superconductivity at 20 K in $Ca_{1-x}Na_xFe_2As_2$,"We report that intrinsic transport and magnetic properties, and their anisotropy from high quality single crystal $CaFe_2As_2$. The resistivity anisotropy ($\rho_c/\rho_{ab}$) is $\sim 50 $, and less than 150 of $BaFe_2As_2$, which arises from the strong coupling along c-axis due to an apparent contraction of about 0.13 nm compared to $BaFe_2As_2$. Temperature independent anisotropy indicates that the transport in ab plane and along c-axis direction shares the same scattering mechanism. In sharp contrast to the case of parent compounds $ROFeAs$ (R=rare earth) and $MFe_2As_2$ (M=Ba and Sr), spin-density-wave (SDW) ordering (or structural transition) leads to a steep increase of resistivity in $CaFe_2As_2$. Such different resistivity response to SDW ordering is helpful to understand the role played by SDW ordering in Fe-based high-$T_c$ superconductors. The susceptibility behavior is very similar to that observed in single crystal $BaFe_2As_2$. A linear temperature dependent susceptibility occurs above SDW transition of about 165 K. Partial substitution of Na for Ca suppresses the SWD ordering (anomaly in resistivity) and induces occurrence of superconductivity at $\sim 20$ K.",0806.4279v1 2014-02-25,Measurement of junction conductance and proximity effect at superconductor/semiconductor junctions,"The superconducting proximity effect has played an important role in recent work searching for Majorana modes in thin semiconductor devices. Using transport measurements to quantify the changes in the semiconductor caused by the proximity effect provides a measure of dynamical processes such as screening and scattering. However, in a two terminal measurement the resistance due to the interface conductance is in series with resistance of transport in the semiconductor. Both of these change, and it is impossible to separate them without more information. We have devised a new three terminal device that provides two resistance measurements that are sufficient to extract both the junction conductance and the two dimensional sheet resistance under the superconducting contact. We have compared junctions between Nb and InAs and Nb and 30% InGaAs all grown before being removed from the ultra high vacuum molecular beam epitaxy growth system. The most transparent junctions are to InAs, where the transmission coefficient per Landauer mode is greater than 0.6. Contacts made with ex-situ deposition are substantially more opaque. We find that for the most transparent junctions, the largest fractional change as the temperature is lowered is to the resistance of the semiconductor.",1402.6055v1 2018-08-14,Impurities and Defects in Mott Systems,"Disorder has intriguing consequences for correlated electronic materials, which include several families of high-temperature superconductors and resistive switching systems. We address the question of why strongly correlated d-wave superconductors, such as the cuprates, prove to be surprisingly robust against the introduction of non-magnetic impurities. We show that, very generally, both the pair-breaking and the normal state transport scattering rates are significantly suppressed by strong correlations effects arising in the proximity to a Mott insulating state. We also show that the correlation-renormalized scattering amplitude is generically enhanced in the forward direction, an effect which was previously often ascribed to the specific scattering by charged impurities outside the copper-oxide planes. We provide the theoretical insights for resistive switching systems and show how impurities and underlying correlations can play significant roles in practical devices. We report the striking result of a connection between the resistive switching and shock wave formation, a classic topic of non-linear dynamics. We argue that the profile of oxygen vacancies that migrate during the commutation forms a shock wave that propagates through a highly resistive region of the device. We validate the scenario by means of model simulations and experiments in a manganese-oxide based memristor device and we extend our theory to the case of binary oxides. The shock wave scenario brings unprecedented physical insight and enables to rationalize the process of oxygen-vacancy-driven resistive change with direct implications for a key technological aspect- the commutation speed.",1808.04767v1 2023-01-10,Microstructuring YbRh2Si2 for resistance and noise measurements down to ultra-low temperatures,"The discovery of superconductivity in the quantum critical Kondo-lattice system YbRh2Si2 at an extremely low temperature of 2 mK has inspired efforts to perform high-resolution electrical resistivity measurements down to this temperature range in highly conductive materials. Here we show that control over the sample geometry by microstructuring using focused-ion-beam (FIB) techniques allows to reach ultra-low temperatures and increase signal-to-noise ratios (SNR) tenfold, without adverse effects to sample quality. In five experiments we show four-terminal sensing resistance and magnetoresistance measurements which exhibit sharp phase transitions at the N\'eel temperature, and Shubnikov-de-Haas (SdH) oscillations between 13 T and 18 T where we identified a new SdH frequency of 0.39 kT. The increased SNR allowed resistance fluctuation (noise) spectroscopy that would not be possible for bulk crystals, and confirmed intrinsic 1/f-type fluctuations. Under controlled strain, two thin microstructured samples exhibited a large increase of T_N from 67 mK up to 188 mK while still showing clear signatures of the phase transition and SdH oscillations. SQUID-based thermal noise spectroscopy measurements in a nuclear demagnetisation refrigerator down to 0.95 mK, show a sharp superconducting transition at T_c = 1.2 mK. These experiments demonstrate microstructuring as a powerful tool to investigate the resistance and the noise spectrum of highly conductive correlated metals over wide temperature ranges.",2301.03928v1 2024-05-06,Bayesian optimization for stable properties amid processing fluctuations in sputter deposition,"We introduce a Bayesian optimization approach to guide the sputter deposition of molybdenum thin films, aiming to achieve desired residual stress and sheet resistance while minimizing susceptibility to stochastic fluctuations during deposition. Thin films are pivotal in numerous technologies, including semiconductors and optical devices, where their properties are critical. Sputter deposition parameters, such as deposition power, vacuum chamber pressure, and working distance, influence physical properties like residual stress and resistance. Excessive stress and high resistance can impair device performance, necessitating the selection of optimal process parameters. Furthermore, these parameters should ensure the consistency and reliability of thin film properties, assisting in the reproducibility of the devices. However, exploring the multidimensional design space for process optimization is expensive. Bayesian optimization is ideal for optimizing inputs/parameters of general black-box functions without reliance on gradient information. We utilize Bayesian optimization to optimize deposition power and pressure using a custom-built objective function incorporating observed stress and resistance data. Additionally, we integrate prior knowledge of stress variation with pressure into the objective function to prioritize films least affected by stochastic variations. Our findings demonstrate that Bayesian optimization effectively explores the design space and identifies optimal parameter combinations meeting desired stress and resistance specifications.",2405.03092v1 2023-04-06,Performance Analysis of DNA Crossbar Arrays for High-Density Memory Storage Applications,"Deoxyribonucleic acid (DNA) has emerged as a promising building block for next-generation ultra-high density storage devices. Although DNA has high durability and extremely high density in nature, its potential as the basis of storage devices is currently hindered by limitations such as expensive and complex fabrication processes and time-consuming read-write operations. In this article, we propose the use of a DNA crossbar array architecture for an electrically readable Read-Only Memory (DNA-ROM). While information can be written error-free to a DNA-ROM array using appropriate sequence encoding, its read accuracy can be affected by several factors such as array size, interconnect resistance, and Fermi energy deviations from HOMO levels of DNA strands employed in the crossbar. We study the impact of array size and interconnect resistance on the bit error rate of a DNA-ROM array through extensive Monte Carlo simulations. We have also analyzed the performance of our proposed DNA crossbar array for an image storage application, as a function of array size and interconnect resistance. While we expect that future advances in bioengineering and materials science will address some of the fabrication challenges associated with DNA crossbar arrays, we believe that the comprehensive body of results we present in this paper establishes the technical viability of DNA crossbar arrays as low-power, high-density storage devices. Finally, our analysis of array performance vis-a-vis interconnect resistance should provide valuable insights into aspects of the fabrication process such as the proper choice of interconnects necessary for ensuring high read accuracies.",2304.14269v1 2023-11-09,Signature of superconductivity in pressurized La$_4$Ni$_3$O$_{10}$,"The discovery of high-temperature superconductivity near 80 K in bilayer nickelate La$_3$Ni$_2$O$_7$ under high pressures has renewed the exploration of superconducting nickelate in bulk materials. The extension of superconductivity in other nickelates in a broader family is also essential. Here, we report the experimental observation of superconducting signature in trilayer nickelate La$_4$Ni$_3$O$_{10}$ under high pressures. By using a modified sol-gel method and post-annealing treatment under high oxygen pressure, we successfully obtained polycrystalline La$_4$Ni$_3$O$_{10}$ samples with different transport behaviors at ambient pressure. Then we performed high-pressure electrical resistance measurements on these samples in a diamond-anvil-cell (DAC) apparatus. Surprisingly, the signature of possible superconducting transition with a maximum transition temperature ($T_\text{c}$) of about 20 K under high pressures is observed, as evidenced by a clear drop of resistance and the suppression of resistance drops under magnetic fields. Although the resistance drop is sample-dependent and relatively small, it appears in all of our measured samples. We argue that the observed superconducting signal is most likely to originate from the main phase of La$_4$Ni$_3$O$_{10}$. Our findings will motivate the exploration of superconductivity in a broader family of nickelates and shed light on the understanding of the underlying mechanisms of high-$T_\text{c}$ superconductivity in nickelates.",2311.05453v1 2024-04-29,Thermoelectric transport properties of the quasi-one-dimensional dimer-Mott insulator $β'$-(BEDT-TTF)$_2$ICl$_2$,"Low-dimensional materials, in which the electronic and transport properties are drastically modified in comparison to those of three-dimensional bulk materials, yield a key class of thermoelectric materials with high conversion efficiency. Among such materials, the organic compounds may serve peculiar properties owing to their unique molecular-based low-dimensional structures with highly anisotropic molecular orbitals. Here we present the thermoelectric transport properties of the quasi-one-dimensional dimer-Mott insulator $\beta'$-(BEDT-TTF)$_2$ICl$_2$, where BEDT-TTF stands for bis(ethylenedithio)-tetrathiafulvalene. We find that the thermopower exhibits typical activation-type temperature variation expected for insulators but its absolute value is anomalously large compared to the expected value from the activation-type temperature dependence of the electrical resistivity. Successively, the Jonker-plot analysis, in which the thermopower is usually scaled by the logarithm of the resistivity, shows an unusual relation among such transport quantities. We discuss a role of the low dimensionality for the enhanced thermopower along with recent observations of such a large thermopower in several low-dimensional materials.",2404.19137v1 2021-12-28,Review of Transition-Metal Diboride Thin Films,"We review the thin film growth, chemistry, and physical properties of Group 4-6 transition-metal diboride (TMB2) thin films with AlB2-type crystal structure (Strukturbericht designation C32). Industrial applications are growing rapidly as TMB2 begin competing with conventional refractory ceramics like carbides and nitrides, including pseudo-binaries such as Ti1-xAlxN. The TMB2 crystal structure comprises graphite-like honeycombed atomic sheets of B interleaved by hexagonal close-packed TM layers. From the C32 crystal structure stems unique properties including high melting point, hardness, and corrosion resistance, yet limited oxidation resistance, combined with high electrical conductivity. We correlate the underlying chemical bonding, orbital overlap, and electronic structure to the mechanical properties, resistivity, and high-temperature properties unique to this class of materials. The review highlights the importance of avoiding contamination elements (like oxygen) and boron segregation on both the target and substrate sides during sputter deposition, for better-defined properties, regardless of the boride system investigated. This is a consequence of the strong tendency for B to segregate to TMB2 grain boundaries for boron-rich compositions of the growth flux. It is judged that sputter deposition of TMB2 films is at a tipping point towards a multitude of applications for TMB2 not solely as bulk materials, but also as protective coatings and electrically conducting high-temperature stable thin films.",2112.14099v1 2016-06-10,On the search for the chiral anomaly in Weyl semimetals: The negative longitudinal magnetoresistance,"Recently, the existence of massless chiral (Weyl) fermions has been postulated in a class of semi-metals with a non-trivial energy dispersion.These materials are now commonly dubbed Weyl semi-metals (WSM).One predicted property of Weyl fermions is the chiral or Adler-Bell-Jackiw anomaly, a chirality imbalance in the presence of parallel magnetic and electric fields. In WSM, it is expected to induce a negative longitudinal magnetoresistance (NMR), the chiral magnetic effect.Here, we present experimental evidence that the observation of the chiral magnetic effect can be hindered by an effect called ""current jetting"". This effect also leads to a strong apparent NMR, but it is characterized by a highly non-uniform current distribution inside the sample. It appears in materials possessing a large field-induced anisotropy of the resistivity tensor, such as almost compensated high-mobility semimetals due to the orbital effect.In case of a non-homogeneous current injection, the potential distribution is strongly distorted in the sample.As a consequence, an experimentally measured potential difference is not proportional to the intrinsic resistance.Our results on the MR of the WSM candidate materials NbP, NbAs, TaAs, TaP exhibit distinct signatures of an inhomogeneous current distribution, such as a field-induced ""zero resistance' and a strong dependence of the `measured resistance"" on the position, shape, and type of the voltage and current contacts on the sample. A misalignment between the current and the magnetic-field directions can even induce a ""negative resistance"". Finite-element simulations of the potential distribution inside the sample, using typical resistance anisotropies, are in good agreement with the experimental findings. Our study demonstrates that great care must be taken before interpreting measurements of a NMR as evidence for the chiral anomaly in putative Weyl semimetals.",1606.03389v1 2011-10-07,Overlapping-gate architecture for silicon Hall bar MOSFET devices in the low electron density and high magnetic field regime,"A common issue in low temperature measurements of enhancement-mode metal-oxide-semiconductor (MOS) field-effect transistors (FETs) in the low electron density regime is the high contact resistance dominating the device impedance. In that case a voltage bias applied across the source and drain contact of a Hall bar MOSFET will mostly fall across the contacts (and not across the channel) and therefore magneto-transport measurements become challenging. However, from a physical point of view, the study of MOSFET nanostructures in the low electron density regime is very interesting (impurity limited mobility [1], carrier interactions [2,3] and spin-dependent transport [4]) and it is therefore important to come up with solutions [5,6] that work around the problem of a high contact resistance in such devices (c.f. Fig. 1 (a)).",1110.1418v1 2013-04-01,"Novel Bismaleimide Resin/Silsesquioxane and Titania Nanocomposites by the Sol-Gel Process: the Preparation, Morphology, Thermal and Thermo-mechanical Properties","Bismaleimide(BMI) resin/silsesquioxane or titania nanocomposites were synthesized from bismaleimide resin and SiO3/2 or TiO2 via the sol-gel process of N-{\gamma}-triethoxylsilylpropyl-maleamic acid (TESPMA) or tetrabutyltitanate (Ti(OnBu)4, TBT), respectively, in the presence of the AP-BMI prepolymers. These nanocomposite materials were characterized by FT-IR, FE-SEM, TGA and DMA. It was found that the nano-scale SiO3/2 or TiO2 particles were formed in the AP-BMI resin matrix and the average original particle size of the dispersed phase in the nanocomposites was less than 100nm, but the particle aggregates with bigger size existed. Obvious improvements of Tg and the heat resistance of the AP-BMI resin were achieved by introduction of the nano-sized SiO3/2 inorganic phase, and the modulus at high temperatures was improved too. The incorporation of nano-scale TiO2 particles into the AP-BMI resin improved the Tg of the polymer, but lowered the thermal resistance of the material, and improved the modulus of the material at lower temperatures, but lowered the modulus at higher temperatures.",1304.0288v1 2016-04-19,Observation of spin Seebeck contribution to the transverse thermopower in Ni-Pt and MnBi-Au bulk nanocomposites,"Transverse thermoelectric devices produce electric fields perpendicular to an incident heat flux. Classically, this process is driven by the Nernst effect in bulk solids, wherein a magnetic field generates a Lorentz force on thermally excited electrons. The spin Seebeck effect (SSE) also produces magnetization-dependent transverse electric fields. SSE is traditionally observed in thin metallic films deposited on electrically insulating ferromagnets, but the films' high resistance limits thermoelectric conversion efficiency. Combining Nernst and SSE in bulk materials would enable devices with simultaneously large transverse thermopower and low electrical resistance. Here we demonstrate experimentally this is possible in composites of conducting ferromagnets (Ni or MnBi) containing metallic nanoparticles with strong spin-orbit interactions (Pt or Au). These materials display positive shifts in transverse thermopower attributable to inverse spin Hall electric fields in the nanoparticles. This more than doubles the power output of the Ni-Pt materials, establishing proof-of-principle that SSE persists in bulk nanocomposites.",1604.05626v3 2016-01-18,Large magnetoresistance in LaBi: origin of field-induced resistivity upturn and plateau in compensated semimetals,"The discovery of non-magnetic extreme magnetoresistance (XMR) materials has induced great interests because the XMR phenomenon challenges our understanding of how a magnetic field can alter electron transport in semimetals. Among XMR materials, the LaSb shows XMR and field-induced exotic behaviors but it seems to lack the essentials for these properties. Here, we study the magnetotransport properties and electronic structure of LaBi, isostructural to LaSb. LaBi exhibits large MR as in LaSb, which can be ascribed to the nearly compensated electron and hole with rather high mobilities. More importantly, our analysis suggests that the XMR as well as field-induced resistivity upturn and plateau observed in LaSb and LaBi can be well explained by the two-band model with the compensation situation. We present the critical conditions leading to these field-induced properties. It will contribute to understanding the XMR phenomenon and explore novel XMR materials.",1601.04618v2 2003-03-14,Microwave performance of high-density bulk MgB2,"We have performed microwave measurements on superconducting hot-isostatically- pressed (HIPed) bulk MgB2 using a parallel-plate resonator technique. The high density and strength of the HIPed material allowed preparation of samples with mirror-like surfaces for microwave measurements. The microwave surface resistance decreased by about 40% at 20 K when the root-mean-square surface roughness was reduced from 220 nm to 110 nm through surface-polishing and ion-milling. The surface resistance was independent of surface microwave magnetic field at least up to 4 Oe and below 30 K. We attribute this behavior, and the overall low surface resistance (~0.8 mOhms at 10 GHz and 20 K), to the high density of our samples and the absence of weak links between grains.",0303283v1 2006-02-23,Quantum Metallicity on the High-Field Side of the Superconductor-Insulator Transition,"We investigate ultrathin superconducting TiN films, which are very close to the localization threshold. Perpendicular magnetic field drives the films from the superconducting to an insulating state, with very high resistance. Further increase of the magnetic field leads to an exponential decay of the resistance towards a finite value. In the limit of low temperatures, the saturation value can be very accurately extrapolated to the universal quantum resistance h/e^2. Our analysis suggests that at high magnetic fields a new ground state, distinct from the normal metallic state occurring above the superconducting transition temperature, is formed. A comparison with other studies on different materials indicates that the quantum metallic phase following the magnetic-field-induced insulating phase is a generic property of systems close to the disorder-driven superconductor-insulator transition.",0602557v2 2013-09-18,Pressure-Induced Superconductivity in Mineral Calaverite AuTe2,"The pressure dependences of resistivity and ac susceptibility have been measured in the mineral calaverite AuTe$_2$. Resistivity clearly shows a first-order phase transition into a high-pressure phase, consistent with the results of a previous structural analysis. We found zero resistivity and a diamagnetic shielding signal at low temperatures in the high-pressure phase, which clearly indicates the appearance of superconductivity. Our experimental results suggest that bulk superconductivity appears only in the high-pressure phase. For AuTe$_2$, the highest superconducting transition temperature under pressure is $T_{\rm c}$ = 2.3 K at 2.34 GPa; it was $T_{\rm c}$ = 4.0 K for Pt-doped (Au$_{0.65}$Pt$_{0.35}$)Te$_2$. The difference in $T_{\rm c}$ between the two systems is discussed on the basis of the results obtained using the band calculations and McMillan's formula.",1309.4827v2 2018-03-07,Saturation and negative temperature coefficient of electrical resistivity in liquid iron-sulfur alloys at high densities from first principles calculations,"We report results on electronic transport properties of liquid Fe-S alloys at conditions of planetary cores, computed by first-principle techniques in the Kubo-Greenwood formalism. We describe a combined effect of resistivity saturation due to temperature, compression, and chemistry by comparing the electron mean free path from the Drude response of optical conductivity to the mean interatomic distance. At high compression and high sulfur concentration the Ioffe-Regel condition is satisfied, and the temperature coefficient of resistivity changes sign from positive to negative. We show that this happens due to a decrease of the $d$-density of states at the Fermi level in response to thermal broadening.",1803.02649v1 2018-10-03,On the temperature scaling behaviour of the linear magnetoresistance observed in high-temperature superconductors,"An analytical model invoking variations in the charge-carrier density is used to generate magnetoresistance curves that are almost indistinguishable from those produced by sophisticated numerical models. This demonstrates that, though disorder is pivotal in causing linear magnetoresistance, the form of the magnetoresistance thus generated is insensitive to details of the disorder. Taken in conjunction with the temperature ($T$) dependence of the zero-field resistivity, realistic levels of disorder are shown to be sufficient to explain the linear magnetoresistance and field-$T$ resistance scaling observed in high-temperature pnictide and cuprate superconductors. Hence, though the $T$-linear zero-field resistance is a definite signature of the ""strange metal"" state of high-temperature superconductors, their linear magnetoresistance and its scaling is unlikely to be so.",1810.01998v3 2020-04-17,High-pressure characterization of multifunctional CrVO4,"The structural stability and physical properties of CrVO4 under compression were studied by X-ray diffraction, Raman spectroscopy, optical absorption, resistivity measurements, and ab initio calculations up to 10 GPa. High-pressure X-ray diffraction and Raman measurements show that CrVO4 undergoes a phase transition from the ambient pressure orthorhombic CrVO4-type structure (Cmcm space group, phase III) to the high-pressure monoclinic CrVO4-V phase, which is isomorphic to the wolframite structure. Such a phase transition (CrVO4-type - wolframite), driven by pressure, also was previously observed in indium vanadate. The crystal structure of both phases and the pressure dependence in unit-cell parameters, Raman-active modes, resistivity, and electronic band gap, is reported. Vanadium atoms are sixth-fold coordinated in the wolframite phase, which is related to the collapse in the volume at the phase transition. Besides, we also observed drastic changes in the phonon spectrum, a drop of the band-gap, and a sharp decrease of resistivity. All the observed phenomena are explained with the help of first-principles calculations.",2004.08072v1 2020-08-28,"High-Bandwidth, Variable-Resistance Differential Noise Thermometry","We develop Johnson noise thermometry applicable to mesoscopic devices with variable source impedance with high bandwidth for fast data acquisition. By implementing differential noise measurement and two-stage impedance matching, we demonstrate noise measurement in the frequency range 120-250 MHz with a wide sample resistance range 30 {\Omega}-100 k{\Omega} tuned by gate voltages and temperature. We employ high-frequency, single-ended low noise amplifiers maintained at a constant cryogenic temperature in order to maintain the desired low noise temperature. We achieve thermometer calibration with temperature precision up to 650 mK on a 10 K background with 30 s of averaging. Using this differential noise thermometry technique, we measure thermal conductivity on a bilayer graphene sample spanning the metallic and semiconducting regimes in a wide resistance range, and we compare it to the electrical conductivity.",2008.12739v1 2014-09-19,Fluorine doping: A feasible solution to enhancing the conductivity of high-resistance wide bandgap Mg0.51Zn0.49O active components,"N-type doping of high-resistance wide bandgap semiconductors, wurtzite high-Mg-content MgxZn1-xO for instance, has always been a fundamental application-motivated research issue. Herein, we report a solution to enhancing the conductivity of high-resistance Mg0.51Zn0.49O active components, which has been reliably achieved by fluorine doping via radio-frequency plasma assisted molecular beam epitaxial growth. Fluorine dopants were demonstrated to be effective donors in Mg0.51Zn0.49O single crystal film having a solar-blind 4.43 eV bandgap, with an average concentration of 1.0E19 F/cm3.The dramatically increased carrier concentration (2.85E17 cm-3 vs ~1014 cm-3) and decreased resistivity (129 ohm.cm vs ~10E6 ohm cm) indicate that the electrical properties of semi-insulating Mg0.51Zn0.49O film can be delicately regulated by F doping. Interestingly, two donor levels (17 meV and 74 meV) associated with F were revealed by temperature-dependent Hall measurements. A Schottky type metal-semiconductor-metal ultraviolet photodetector manifests a remarkably enhanced photocurrent, two orders of magnitude higher than that of the undoped counterpart. The responsivity is greatly enhanced from 0.34 mA/W to 52 mA/W under 10 V bias. The detectivity increases from 1.89E9 cm Hz1/2/W to 3.58eE10 cm Hz1/2/W under 10 V bias at room temperature.These results exhibit F doping serves as a promising pathway for improving the performance of high-Mg-content MgxZn1-xO-based devices.",1409.5657v2 2021-11-03,Resistive switching in HfO2-x/La0.67Sr0.33MnO3 heterostructure: An intriguing case of low H-field susceptibility of an E-field controlled active interface,"High-performance non-volatile resistive random access memories (ReRAM) and their small stimuli control are of immense interest for high-speed computation and big-data processing in the emergent Internet of Things (IOT) arena. Here, we examine the resistive switching (RS) behavior in growth controlled HfO2/La0.67Sr0.33MnO3 heterostructures and their tunability under low magnetic field. It is demonstrated that oxygen-deficient HfO2 films show bipolar switching with high on/off ratio, stable retention, as well as good endurance owing to the orthorhombic-rich phase constitution and charge (de)-trapping-enabled Schottky-type conduction. Most importantly, we have demonstrated that, the RS can be tuned by a very low externally applied magnetic field (0-30 mT). Remarkably, application of a magnetic field of 30 mT causes the RS to be fully quenched and frozen in the high resistance state (HRS) even after the removal of magnetic field. However, the quenched state could be resurrected by applying higher bias voltage than the one for initial switching. This is argued to be a consequence of the electronically and ionically active nature of the HfO2-x/LSMO interface on both sides, and its susceptibility to the electric and low magnetic field effects. This result could pave the way for new designs of interface engineered high-performance oxitronic ReRAM devices.",2111.02476v1 2002-09-26,Kapitza resistance at the liquid solid interface,"Using equilibrium and nonequilibrium molecular dynamics simulations, we determine the Kapitza resistance (or thermal contact resistance) at a model liquid solid interface. The Kapitza resistance (or the associated Kapitza length) can reach appreciable values when the liquid does not wet the solid. The analogy with the hydrodynamic slip length is discussed.",0209607v1 2008-02-06,On the calculation of Schottky contact resistivity,"This numerical study examines the importance of self-consistently accounting for transport and electrostatics in the calculaiton of semiconductor/metal Schottky contact resistivity. It is shown that ignoring such self-consistency results in significant under-estimation of the contact resistivity. An explicit numerical method has also been proposed to efficiently improve contact resistivity calculations.",0802.0729v1 2016-12-17,"Upper critical field, pressure-dependent superconductivity and electronic anisotropy of Sm$_4$Fe$_2$As$_2$Te$_{1-x}$O$_{4-y}$F$y$","We present a detailed study of the electrical transport properties of a recently discovered iron-based superconductor: Sm$_4$Fe$_2$As$_2$Te$_{0.72}$O$_{2.8}$F$_{1.2}$. We followed the temperature dependence of the upper critical field by resistivity measurement of single crystals in magnetic fields up to 16 T, oriented along the two main crystallographic directions. This material exhibits a zero-temperature upper critical field of 90 T and 65 T parallel and perpendicular to the Fe$_2$As$_2$ planes, respectively. An unprecedented superconducting magnetic anisotropy $\gamma_H=H_{c2}^{ab}/H_{c2}^c \sim 14$ is observed near Tc, and it decreases at lower temperatures as expected in multiband superconductors. Direct measurement of the electronic anisotropy was performed on microfabricated samples, showing a value of $\rho_c/\rho_{ab}(300K) \sim 5$ that raises up to 19 near Tc. Finally, we have studied the pressure and temperature dependence of the in-plane resistivity. The critical temperature decreases linearly upon application of hydrostatic pressure (up to 2 GPa) similarly to overdoped cuprate superconductors. The resistivity shows saturation at high temperatures, suggesting that the material approaches the Mott-Ioffe-Regel limit for metallic conduction. Indeed, we have successfully modelled the resistivity in the normal state with a parallel resistor model that is widely accepted for this state. All the measured quantities suggest strong pressure dependence of the density of states.",1612.05792v1 2019-07-28,Field-dependent nonlinear surface resistance and its optimization by surface nano-structuring in superconductors,"We propose a theory of nonlinear surface resistance of a dirty superconductor in a strong radio-frequency (RF) field, taking into account magnetic and nonmagnetic impurities, finite quasiparticle lifetimes, and a thin proximity-coupled normal layer characteristic of the oxide surface of many materials. The Usadel equations were solved to obtain the quasiparticle density of states (DOS) and the low-frequency surface resistance $R_s$ as functions of the RF field amplitude $H_0$. It is shown that the interplay of the broadening of the DOS peaks and a decrease of a quasiparticle gap caused by the RF currents produces a minimum in $R_s(H_0)$ and an extended rise of the quality factor $Q(H_0)$ with the RF field. Paramagnetic impurities shift the minimum in $R_s(H_0)$ to lower fields and can reduce $R_s(H_0)$ in a wide range of $H_0$. Subgap states in the DOS can give rise to a residual surface resistance while reducing $R_s$ at higher temperatures. A proximity-coupled normal layer at the surface can shift the minimum in $R_s(H_0)$ to either low and high fields and can reduce $R_s$ below that of an ideal surface. The theory shows that the behavior of $R_s(H_0)$ changes as the temperature and the RF frequency are increased, and the field dependence of $Q(H_0)$ can be very sensitive to the materials processing. Our results suggest that the nonlinear RF losses can be minimized by tuning pairbreaking effects at the surface using impurity management or surface nanostructuring.",1907.12040v1 2019-08-08,Substrate induced nanoscale resistance variation in epitaxial graphene,"Graphene, the first true two-dimensional material still reveals the most remarkable transport properties among the growing class of two-dimensional materials. Although many studies have investigated fundamental scattering processes, the surprisingly large variation in the experimentally determined resistances associated with a localized defect is still an open issue. Here, we quantitatively investigate the local transport properties of graphene prepared by polymer assisted sublimation growth (PASG) using scanning tunneling potentiometry. PASG graphene is characterized by a spatially homogeneous current density, which allows to analyze variations in the local electrochemical potential with high precision. We utilize this possibility by examining the local sheet resistance finding a significant variation of up to 270% at low temperatures. We identify a correlation of the sheet resistance with the stacking sequence of the 6H-SiC substrate as well as with the distance between the graphene sheet and the substrate. Our results experimentally quantify the strong impact of the graphene-substrate interaction on the local transport properties of graphene.",1908.02956v2 2021-01-16,Optical Tuning of Resistance Switching in Polycrystalline Gallium Phosphide Thin Films,"The nanoscale resistive switching characteristics of gallium phosphide (GaP) thin films directly grown on Si are investigated as a function of incident light. Firstly, as-grown GaP films show a high RON/ROFF (~10^4), shown to arise from the formation of conductive channels along the grain boundaries. It is proposed that point defects (most likely Ga interstitials) and structural disorder at the grain boundaries provide the ideal environment to enable the filamentary switching process. Next, we explored if such defects can give rise to mid-gap states, and if so could they be activated by photonic excitation. Both first-principles calculations as well as UV-vis and photoluminescence spectroscopy strongly point to the possibility of mid-gap electronic states in the polycrystalline GaP film. Photoconductive atomic force microscopy (phAFM), a scanning probe technique, is used to image photocurrents generated as a function of incident photon energy (ranging from sub band-gap to above band-gap) on the GaP film surface. We observe photocurrents even for incident photon energies lower than the band-gap, consistent with the presence of mid-gap electronic states. Moreover the photocurrent magnitude is found to be directly proportional to the incident photon energy with a concomitant decrease in the filament resistance. This demonstrates GaP directly integrated on Si can be a promising photonic resistive switching materials system.",2101.06538v1 2020-11-03,Switchable domains in point contacts based on transition metal tellurides,"We report resistive switching in voltage biased point contacts (PCs) based on series of van der Waals transition metals tellurides (TMTs) such as MeTe2 (Me=Mo, W) and TaMeTe4 (Me= Ru, Rh, Ir). The switching occurs between a low resistive ""metallic-type"" state, which is the ground state, and a high resistive ""semiconducting-type"" state by applying certain bias voltage (<1V), while reverse switching takes place by applying voltage of opposite polarity. The origin of the effect can be formation of domain in PC core by applying a bias voltage, when a strong electric field (about 10kV/cm) modifies the crystal structure and controls its polarization. In addition to the discovery of the switching effect in PCs, we also suggest a simple method of material testing before functionalizing them, which offers a great advantage in finding suitable novel substances. The new functionality of studied TMTs arising from switchable domains in submicron hetero-structures that are promising, e.g., for non-volatile resistive random access memory (RRAM) engineering.",2011.01569v2 2020-11-30,Above-room-temperature giant thermal conductivity switching in spintronic multilayer,"Thermal switching provides an effective way for active heat flow control, which has recently attracted increasing attention in terms of nanoscale thermal management technologies. In magnetic and spintronic materials, the thermal conductivity depends on the magnetization configuration: this is the magneto-thermal resistance effect. Here we show that an epitaxial Cu/Co$_{50}$Fe$_{50}$ multilayer film exhibits giant magnetic-field-induced modulation of the cross-plane thermal conductivity. The magneto-thermal resistance ratio for the Cu/Co$_{50}$Fe$_{50}$ multilayer reaches 150% at room temperature, which is much larger than the previous record high. Although the ratio decreases with increasing the temperature, the giant magneto-thermal resistance effect of ~100% still appears up to 400 K. The magnetic field dependence of the thermal conductivity of the Cu/Co$_{50}$Fe$_{50}$ multilayer was observed to be about twice greater than that of the cross-plane electrical conductivity. The observation of the giant magneto-thermal resistance effect clarifies a potential of spintronic multilayers as thermal switching devices.",2011.14558v1 2022-03-01,Cu-doping effects on the ferromagnetic semimetal CeAuGe,"We present a study of Cu-substitution effects in 4f-Ce intermetallic compound CeAu1-xCuxGe, with potentially unusual electronic states, in the whole concentration range (x = 0.0 - 1.0). The parent CeAuGe compound, crystallizing in a non-centrosymmetric hexagonal structure, is a ferromagnetic semimetal with Curie temperature 10 K. Cu-doping on Au-site of CeAuGe, CeAu1-xCuxGe, changes the crystal structure from the non-centrosymmetric (P63mc) to centrosymmetric (P63/mmc) space group at the concentration x ~ 0.5, where the c-lattice constant has a maximum value. Magnetic susceptibility and electrical resistivity measurements reveal that all Cu-doped compounds undergo magnetic phase transition near 10 K, with the maximum transition temperature of 12 K for x = 0.5. The neutron powder diffraction experiments show the ferromagnetic ordering of Ce3+ magnetic moments with a value of ~ 1.2 Bohr magneton at 1.8 K, oriented perpendicular to the hexagonal c-axis. By using symmetry analysis, we have found the solutions for the magnetic structure in the ferromagnetic Shubnikov space groups Cmc'21' and P21'/m' for x < 0.5 and x >= 0.5, respectively. Electrical resistivity exhibits a metallic temperature behaviour in all compounds. The resistivity has a local minimum in the paramagnetic state due to Kondo effects at high doping x = 0.8 and 1.0. At the small Cu-doping level, x = 0.2, the resistivity shows a broad feature at the ferromagnetic transition temperature and an additional transition-like peculiarity at 2.5 K in the ferromagnetic state.",2203.00335v1 2022-06-13,The two-dimensional metallic triangular lattice antiferromagnet CeCd3P3,"Single crystals of $R$Cd$_{3}$P$_{3}$ ($R$ = La and Ce) have been investigated by magnetization, electrical resistivity, Hall coefficient, and specific heat. Magnetization measurements of CeCd$_{3}$P$_{3}$ demonstrate clear quasi-2D magnetic behavior. Electrical resistivity and Hall coefficient measurements suggest that $R$Cd$_{3}$P$_{3}$ compounds are low carrier density metallic systems, in strong contrast to an earlier study of polycrystalline material. Specific heat and electrical resistivity measurements of CeCd$_{3}$P$_{3}$ reveal a high temperature (structural) phase transition at $T_{s} = 127$~K and antiferromagnetic ordering below $T_{N} = 0.41$~K. Upon applying magnetic field in the easy-plane ($H {\parallel} ab$) the magnetic ordering temperature increases to 0.43~K at $H \sim 15$~kOe, demonstrating partial lifting of the magnetic frustration. The large electronic specific heat persists in an unusually wide range of temperature above $T_{N}$, due to the frustrated spins. The observation of conventional metallic behavior in the electrical resistivity suggests that the $f$-electrons in CeCd$_{3}$P$_{3}$ undergo negligible hybridization with the conduction electrons. Thus, CeCd$_{3}$P$_{3}$ may be a model system for exploring the complex interplay between magnetic frustration and RKKY physics on a low carrier density Ce triangular lattice.",2206.06366v1 2023-01-13,Image-Force Barrier Lowering of Schottky Barriers in Two-Dimensional Materials as a Function of Metal Contact Angle,"Two-dimensional (2D) semiconductors are a promising solution for the miniaturization of electronic devices and for the exploration of novel physics. However, practical applications and demonstrations of physical phenomena are hindered by high Schottky barriers at the contacts to 2D semiconductors. While the process of image-force barrier lowering (IFBL) can considerably decrease the Schottky barrier, IFBL is not fully understood for the majority of prevalent contact geometries. We introduce a novel technique to determine the IFBL potential energy with application spanning far beyond that of any existing method. We do so by solving Poisson's equation with the boundary conditions of two metal surfaces separated by an angle Omega. We then prove that our result can also be obtained with the method of images provided a non-Euclidean, cone-manifold space is used. The resulting IFBL is used to calculate the expected contact resistance of the most prevalent geometric contacts. Finally, we investigate contact resistance and show how the stronger IFBL counteracts the effect of larger depletion width with increasing contact angle. We find that top contacts experience lower contact resistance than edge contacts. Remarkably, our results identify tunable parameters for reducing Schottky barriers and likewise contact resistance to edge-contacted 2D materials, enhancing potential applications.",2301.05373v2 2023-12-07,Demonstration of high-impedance superconducting NbRe Dayem bridges,"Here we demonstrate superconducting Dayem-bridge weak-links made of different stoichiometric compositions of NbRe. Our devices possess a relatively high critical temperature, normal-state resistance, and kinetic inductance. In particular, the high kinetic inductance makes this material a good alternative to more conventional niobium-based superconductors (e.g., NbN or NbTiN) for the realization of superinductors and high-quality factor resonators, whereas the high normal-state resistance yields a large output voltage in superconducting switches and logic elements realized upon this compound. Moreover, out-of-plane critical magnetic fields exceeding 2 T ensure that possible applications requiring high magnetic fields can also be envisaged. Altogether, these features make this material appealing for a number of applications in the framework of quantum technologies.",2312.04331v2 2019-01-11,"A Piezoelectric, Strain-Controlled Antiferromagnetic Memory Insensitive to Magnetic Fields","Spintronic devices based on antiferromagnetic (AFM) materials hold the promise of fast switching speeds and robustness against magnetic fields. Different device concepts have been predicted and experimentally demonstrated, such as low-temperature AFM tunnel junctions that operate as spin-valves, or room-temperature AFM memory, for which either thermal heating in combination with magnetic fields, or N\'eel spin-orbit torque is used for the information writing process. On the other hand, piezoelectric materials were employed to control magnetism by electric fields in multiferroic heterostructures, which suppresses Joule heating caused by switching currents and may enable low energy-consuming electronic devices. Here, we combine the two material classes to explore changes of the resistance of the high-N\'eel-temperature antiferromagnet MnPt induced by piezoelectric strain. We find two non-volatile resistance states at room temperature and zero electric field, which are stable in magnetic fields up to 60 T. Furthermore, the strain-induced resistance switching process is insensitive to magnetic fields. Integration in a tunnel junction can further amplify the electroresistance. The tunneling anisotropic magnetoresistance reaches ~11.2% at room temperature. Overall, we demonstrate a piezoelectric, strain-controlled AFM memory which is fully operational in strong magnetic fields and has potential for low-energy and high-density memory applications.",1901.03551v1 2020-07-09,Frequency domain measurements of thermal properties using 3omega-Scanning Thermal Microscope in a vacuum environment,"Material thermal properties characterization at nanoscales remains a challenge even if progresses were done in developing specific characterization techniques like the Scanning Thermal Microscopy (SThM). In the present work, we propose a detailed procedure based on the combined use of a SThM probe characterization and its Finite Element Modeling (FEM) to recover in-operando 3omega measurements achieved under high vacuum. This approach is based on a two-step methodology: (i) a fine description of the probe s electrical and frequency behaviors in out of contact mode to determine intrinsic parameters of the SThM tip, (b) a minimization of the free parameter of our model, i.e. the contact thermal resistance, by comparing 3omega measurements to our simulations of the probe operating in contact mode. Such an approach allows us to accurately measure thermal interface resistances of the probe as a function of the strength applied between the tip and the surface for three different materials (silicon, silica and gold). In addition, FEM modeling provides insights about the 3omega-SThM technique sensitivity, as a function of probe / sample interface resistance to measure material thermal conductivity, paving the way to quantitative SThM measurements.",2007.04632v1 2022-04-02,Traction of Interlocking Spikes on a Granular Material,"The interlock drive system generates traction by inserting narrow articulated spikes into the ground and by leveraging the soil's strength to resist horizontal draft forces. The system promises high tractive performance in low gravity environments where tires have little traction for lack of weight. At Earth and Space 2021 we reported the performance of such spikes on a silty clay loam, a cohesive soil. We found that in such soil, traction below a critical depth is provided by a zone of lateral soil failure. We also found that the articulation translates a horizontal draft force into a vertical penetration force strong enough to penetrate a narrow spike to a depth where the soil can sustain the draft force, in a self-regulating way. It is conceivable that a granular material like regolith or sand with little to no cohesive strength provides less vertical penetration resistance and less resistance to a horizontal draft force than a cohesive soil, which leads to the question of whether and how much tractive force an interlocking spike can generate on a granular material. Here we report on field trials that study different spike designs in dry and unsaturated moist sand. The results demonstrate that a loose granular material requires larger spikes than a cohesive soil, that these larger spikes penetrate dry and moist sand reliably, and that they promise good tractive efficiency. The trials indicate that on sand, a larger spike diameter can improve the pull/weight ratio without a loss of tractive performance.",2205.00840v2 2015-02-12,RF Transport Electromagnetic Properties of CVD Graphene from DC to 110 MHz,"We report measurement of the radio-frequency (RF) transport electromagnetic properties of chemical vapour deposition (CVD) graphene over the DC to 110 MHz frequency range at room temperature. Graphene on Si/SiO2 substrate was mounted in a shielded four terminal-pair (4TP) adaptor which enabled direct connection to a calibrated precision impedance analyser for measurements. Good agreement is observed for the DC four-probe resistance and the 4TP resistance at 40 Hz, both yielding R ~ 104 {\Omega}. In general the apparent graphene channel electromagnetic properties are found to be strongly influenced by the substrate parasitic capacitance and resistance, particularly for high-frequencies f > 1 MHz. A phenomenological lumped-parameter equivalent circuit model is presented which matches the frequency response of the graphene 4TP impedance device over approximately seven decades of the frequency range of the applied transport alternating current. Based on this model, it is shown for the first time, that the intrinsic graphene channel resistance of the 4TP device is frequency-independent (i.e. dissipationless) with RG ~ 105 {\Omega} or sheet resistance of approximately 182 {\Omega} / sq. The parasitic substrate impedance of the device is found shunt RG with RP ~ 2.2 {\Omega} in series with CP ~ 600 pF. These results suggest that our new RF 4TP method is in good agreement with the conventional DC four-probe method for measuring the intrinsic sheet resistance of single-atom thick materials and could potentially open up new applications in RF electronics, AC quantum Hall effect metrology and sensors based on graphene 4TP devices operating over broad range of frequencies.",1502.03835v1 2015-12-11,Intrinsic high electrical conductivity of stoichiometric SrNbO3 epitaxial thin films,"SrVO3 and SrNbO3 are perovskite-type transition-metal oxides with the same d1 electronic configuration. Although SrNbO3 (4d1) has a larger d orbital than SrVO3 (3d1), the reported electrical resistivity of SrNbO3 is much higher than that of SrVO3, probably owing to nonstoichiometry. In this paper, we grew epitaxial, high-conductivity stoichiometric SrNbO3 using pulsed laser deposition. The growth temperature strongly affected the Sr/Nb ratio and the oxygen content of the films, and we obtained stoichiometric SrNbO3 at a very narrow temperature window around 630 ${\deg}$C. The stoichiometric SrNbO3 epitaxial thin films grew coherently on KTaO3 (001) substrates with high crystallinity. The room-temperature resistivity of the stoichiometric film was $2.82 {\times} 10^{-5} {\Omega}$cm, one order of magnitude lower than the lowest reported value of SrNbO3 and comparable with that of SrVO3. We observed a T-square dependence of resistivity below $T^{\ast}$ = 180 K and non-Drude behavior in near-infrared absorption spectroscopy, attributable to the Fermi-liquid nature caused by electron correlation. Analysis of the T-square coefficient A of resistivity experimentally revealed that the 4d orbital of Nb that is larger than the 3d ones certainly contributes to the high electrical conduction of SrNbO3.",1512.03588v1 2020-08-22,Indium-Tin-Oxide Transistors with One Nanometer Thick Channel and Ferroelectric Gating,"In this work, we demonstrate high performance indium-tin-oxide (ITO) transistors with the channel thickness down to 1 nm and ferroelectric Hf0.5Zr0.5O2 as gate dielectric. On-current of 0.243 A/mm is achieved on sub-micron gate-length ITO transistors with a channel thickness of 1 nm, while it increases to as high as 1.06 A/mm when the channel thickness increases to 2 nm. A raised source/drain structure with a thickness of 10 nm is employed, contributing to a low contact resistance of 0.15 {\Omega}mm and a low contact resistivity of 1.1{\times}10-7 {\Omega}cm2. The ITO transistor with a recessed channel and ferroelectric gating demonstrates several advantages over 2D semiconductor transistors and other thin film transistors, including large-area wafer-size nanometer thin film formation, low contact resistance and contact resistivity, atomic thin channel being immunity to short channel effects, large gate modulation of high carrier density by ferroelectric gating, high-quality gate dielectric and passivation formation, and a large bandgap for the low-power back-end-of-line (BEOL) CMOS application.",2008.09881v1 2022-12-13,Collapse of Metallicity and High-$T_c$ Superconductivity in the High-Pressure phase of FeSe$_{0.89}$S$_{0.11}$,"We investigate the high-pressure phase of the iron-based superconductor FeSe$_{0.89}$S$_{0.11}$ using transport and tunnel diode oscillator studies. We construct detailed pressure-temperature phase diagrams that indicate that outside of the nematic phase, the superconducting critical temperature reaches a minimum before it is quickly enhanced towards 40 K above 4 GPa. The resistivity data reveal signatures of a fan-like structure of non-Fermi liquid behaviour which could indicate the existence of a putative quantum critical point buried underneath the superconducting dome around 4.3 GPa. Further increasing the pressure, the zero-field electrical resistivity develops a non-metallic temperature dependence and the superconducting transition broadens significantly. Eventually, the system fails to reach a fully zero-resistance state despite a continuous finite superconducting transition temperature, and any remaining resistance at low temperatures becomes strongly current-dependent. Our results suggest that the high-pressure, high-$T_c$ phase of iron chalcogenides is very fragile and sensitive to uniaxial effects of the pressure medium, cell design and sample thickness which can trigger a first-order transition. These high-pressure regions could be understood assuming a real-space phase separation caused by concomitant electronic and structural instabilities.",2212.06824v1 2023-03-30,Highly tunable NbTiN Josephson junctions fabricated with focused helium ion beam,"We demonstrate a ""direct writing"" method for the fabrication of planar Josephson junctions from high quality superconducting niobium titanium nitride (NbTiN) thin films using focused He-ion beam irradiation. Compared to the materials previously used in such processing, YBCO and MgB$_2$, NbTiN has much better mechanical and electrical properties, as well as good corrosion resistance. We show that we can control the suppression of superconductivity in NbTiN as a function of the helium ion beam fluence, and that this controllable critical temperature suppression combined with the high spatial resolution and position control of the He-ion beam in a helium ion microscope enables us to successfully fabricate Josephson junctions with highly tunable weak links. Because of the continuous nature of the disorder-induced metal-insulator transition, this method allows the creation of barriers with wide range of resistivities ranging from the metallic to the insulating state, with the critical current and the junction resistance varying over two orders of magnitude. Electrical transport measurements show that junctions follow closely the ideal resistively and capacitively shunted junction behavior, have high characteristic voltages ($0.2-1.4$ mV) and show Shapiro steps up to very high orders. This suggests that these type of junctions are suitable for a wide range of applications in superconducting electronics and quantum information technology, with the bonus that a whole device can be fabricated from just a single thin film, with the excellent electrical and microwave characteristics offered by NbTiN.",2303.17348v1 2020-09-05,Corrosion Resistance of Sulfur-Selenium Alloy Coatings,"Despite decades of research, metallic corrosion remains a long-standing challenge in many engineering applications. Specifically, designing a material that can resist corrosion both in abiotic as well as biotic environments remains elusive. Here we design a lightweight sulfur-selenium (S-Se) alloy with high stiffness and ductility that can serve as a universal corrosion-resistant coating with protection efficiency of ~99.9% for steel in a wide range of diverse environments. S-Se coated mild steel shows a corrosion rate that is 6-7 orders of magnitude lower than bare metal in abiotic (simulated seawater and sodium sulfate solution) and biotic (sulfate-reducing bacterial medium) environments. The coating is strongly adhesive and mechanically robust. We attribute the high corrosion resistance of the alloy in diverse environments to its semi-crystalline, non-porous, anti-microbial, and viscoelastic nature with superior mechanical performance, enabling it to successfully block a variety of diffusing species.",2009.02451v1 2006-09-08,Peak resistance temperature and low temperature resistivity in thin film $La_{1-x} Ca_x Mn O_3$ mixtures for x <= 1/3,"The electrical resistivity of La$_{1-x}$Ca$_{x}$MnO$_{3}$ thin films grown on (001) NdGaO$_{3}$ and (100) SrTiO$_{3}$ substrates by off-axis sputtering has been studied as a function of the Calcium doping level. The samples have very narrow rocking curves and excellent in plane registry with the substrate. A strong correlation between the peak resistance temperature and the polaronic hopping energy is seen which is not simply linear. The low temperature resistivity is seen to be fit better by a model of single magnon scattering, and a near linear correlation between the resistivity due to magnon scattering and static impurities is observed.",0609206v1 2011-10-18,Superior performance of multilayered fluoropolymer films in low voltage electrowetting,"The requirement for low operational voltage in electrowetting devices, met using thin dielectrics, is usually connected with serious material failure issues. Dielectric breakdown (visible as electrolysis) is frequently evident slightly beyond the onset of the contact angle saturation. Here, plasma enhanced chemical vapor deposition (PECVD) is used to deposit thin fluorocarbon films prior to the spin-coating of Teflon\textregistered amorphous fluoropolymer on tetraethoxysilane (TEOS) substrates. The resulting multilayered hydrophobic top coating improves the electrowetting performance of the stack, by showing high resistance to dielectric breakdown at high applied voltages and for continuous long term application of DC and AC voltage. Leakage current measurements during electrowetting experiments with the proposed composite coating showed that current remains fairly constant at consecutive electrowetting tests in contrast to plain Teflon\textregistered coating in which material degradation is evident by a progressive increase of the leakage current after multiple electrowetting tests. Since the proposed composite coating demonstrates increased resistance to material failure and to dielectric breakdown even at thin configurations, its integration in electrowetting devices may impact their reliability, robustness and lifetime.",1110.4075v1 2023-12-11,High-speed sensing of RF signals with phase change materials,"RF radiation spectrum is central to wireless and radar systems among numerous high-frequency device technologies. Here, we demonstrate sensing of RF signals in the technologically relevant 2.4 GHz range utilizing vanadium dioxide (VO2), a quantum material that has garnered significant interest for its insulator-to-metal transition. We find the electrical resistance of both stoichiometric as well as off-stoichiometric vanadium oxide films can be modulated with RF wave exposures from a distance. The response of the materials to the RF waves can be enhanced by either increasing the power received by the sample or reducing channel separation. We report a significant ~73% drop in resistance with a 5 {\mu}m channel gap of the VO2 film at a characteristic response time of 16 microseconds. The peak sensitivity is proximal to the phase transition temperature boundary that can be engineered via doping and crystal chemistry. Dynamic sensing measurements highlight the films' rapid response and broad-spectrum sensitivity. Engineering electronic phase boundaries in correlated electron systems could offer new capabilities in emerging communication technologies.",2312.06459v1 2015-09-14,Torsional chiral magnetic effect in Weyl semimetal with topological defect,"We propose a torsional response raised by lattice dislocation in Weyl semimetals akin to chiral magnetic effect; i.e. a fictitious magnetic field arising from screw or edge dislocation induces charge current. We demonstrate that, in sharp contrast to the usual chiral magnetic effect which vanishes in real solid state materials, the torsional chiral magnetic effect exists even for realistic lattice models, which implies the experimental detection of the effect via SQUID or nonlocal resistivity measurements in Weyl semimetal materials.",1509.03981v3 2016-05-02,Study of glass properties as electrode for RPC,"Operation and performance of the Resistive Plate Chambers (RPCs) mostly depend on the quality and characteristics of the electrode materials. The India-based Neutrino Observatory collaboration has chosen glass RPCs as the active detector elements for its Iron Calorimeter detector and is going to deploy RPCs in an unprecedented scale. Therefore, it is imperative that we study the electrode material aspects in detail. We report here, systematic characterization studies on the glasses from two manufacturers. RPC detectors were built using these glasses and performances of the same were compared with their material properties.",1605.01044v1 2010-07-06,Effects of chemical substitution on transport properties of Bi-based high temperature superconductors,"This report describes some transport and magnetic properties of doped Bi2212 and Bi2223 superconducting whiskers. These materials have advantages over polycrystalline sample as well as large bulk crystals in that they provide narrow transitions in resistance versus temperature as well as in magnetization versus temperature curves. In addition they are easy to grow and and have short oxygen annealing times. Here Data on transport and magnetic properties of these superconducting whiskers are presented.",1007.0971v1 2021-07-03,Thin film of Al-Ga-Pd-Mn quasicrystalline alloy,"Thin film quasicrystal coatings have unique properties such as very high electrical and thermal resistivity and very low surface energy. A nano quasicrystalline thin film of icosahedral Al-Ga-Pd-Mn alloy, has produced by flash evaporation followed by annealing. Attempts will be made to discuss the micromechanisms for the formation of quasicrystalline thin film in Al-Ga-Pd-Mn alloys",2107.01478v1 2014-03-06,"Normalized Contact Force to Minimize ""Electrode-Lead"" Resistance in a Nanodevice","In this report, the contact resistance between ""electrode"" and ""lead"" is investigated for reasonable measurements of samples' resistance in a polypyrrole (PPy) nanowire device. The sample's resistance, including ""electrode-lead"" contact resistance, shows a decrease as force applied to the interface increases. Moreover, the sample's resistance becomes reasonably similar to, or lower than, values calculated by resistivity of PPy reported in previous studies. The decrease of electrode-lead contact resistance by increasing the applying force was analyzed by using Holm theory: the general equation of relation between contact resistance ($R_H$) of two-metal thin films and contact force ($R_H$ $\propto$ $1/\sqrt{F}$). The present investigation can guide a reliable way to minimize electrode-lead contact resistance for reasonable characterization of nanomaterials in a microelectrode device.",1403.1357v1 2004-11-12,Microwave induced resistance oscillations on a high-mobility 2DEG: absorption/reflection and temperature damping experiments,"In this work we address experimentally a number of unresolved issues related to microwave induced resistance oscillations (MIRO) and the zero-resistance states observed recently on very high-mobility 2D electron gases in GaAs/AlGaAs heterostructures. In particular, we examine electrodynamic effects via reflection/absorption experiments and study the exact waveform of MIRO and their damping due to temperature. It is shown that electrodynamic effects due to metallic-like reflection and plasmons are important producing a wide cyclotron resonance line and a number of oscillations which do not coincide with the MIRO. To describe the MIRO waveform a simple model was employed involving radiation-induced scattering with displacement. A very good correlation was found between the temperature dependencies of the quantum lifetime from MIRO and the transport scattering time from the electron mobility. The results are compared with measurements of Shubnikov-de Haas oscillations down to 30 mK on the same sample.",0411338v1 2007-04-20,Photoelectric phenomena in structures based on high-resistivity semiconductor crystals with a thin insulator layer at the semiconductor-metal boundary,"A previously unknown effect-giant spatial redistribution of the electric field strength in a crystal under illumination of the structure - was discovered and investigated in real photoresistors on high-resistivity (semi-insulating) semiconductor CdTe crystals (in metal-thin insulator- semiconductor-thin insulator -metal structures). A new concept is proposed for photoelectric phenomena in high- resistivity semiconductor crystals. The concept is based on the idea that the redistribution of the field under such conditions that the carrier lifetime remains unchanged under illumination plays a determining role in these phenomena. The nature of the effect is described, the dependence of the characteristics of the structures on the parameters of the crystal and the insulator layers is explained by the manifestation of this effect, and ways to produce structures with prescribed photoelectric characteristics for new devices and scientific methods are examined.",0704.2703v1 2009-03-15,Current-induced electroresistance in Nd0.5Ca0.5Mn0.95Ni0.05O3,"We have investigated the dc and pulsed current-induced electroresistance in phase separated manganite Nd0.5Ca0.5Mn0.95Ni0.05O3 (NCMONi05) as a function of temperature and magnetic field. It is shown that the negative differential resistance which appears above a threshold current (Ic) and hysteresis in the V-I progressively vanish with increasing period of the current pulses. However a strong non-linearity in V-I exists even for a pulse period of 6s. The peak voltage at Ic decreases in magnitude and shifts towards higher current values with increasing strength of the magnetic field. The strong nonlinear behavior and the negative differential resistance in the dc current sweep are accompanied by a rapid increase of the sample surface temperature and therefore primarily arise from the Joule heating in the sample. While the Joule heating assists electroresistance in the high dc current regime, the nonlinearity in the pulsed current sweep and the resistivity switching between a high and low value induced by controlling the width and period of pulses can not be explained solely on the basis of Joule heating.",0903.2616v2 2009-09-15,Broken symmetry states and divergent resistance in suspended bilayer graphene,"Graphene [1] and its bilayer have generated tremendous excitement in the physics community due to their unique electronic properties [2]. The intrinsic physics of these materials, however, is partially masked by disorder, which can arise from various sources such as ripples [3] or charged impurities [4]. Recent improvements in quality have been achieved by suspending graphene flakes [5,6], yielding samples with very high mobilities and little charge inhomogeneity. Here we report the fabrication of suspended bilayer graphene devices with very little disorder. We observe fully developed quantized Hall states at magnetic fields of 0.2 T, as well as broken symmetry states at intermediate filling factors $\nu = 0$, $\pm 1$, $\pm 2$ and $\pm 3$. The devices exhibit extremely high resistance in the $\nu = 0$ state that grows with magnetic field and scales as magnetic field divided by temperature. This resistance is predominantly affected by the perpendicular component of the applied field, indicating that the broken symmetry states arise from many-body interactions.",0909.2883v1 2010-03-06,Reduction of high reset currents in unipolar resistance switching Pt/SrTiOx/Pt capacitors using acceptor doping,"The high reset current, IR, in unipolar resistance switching is an important issue which should be resolved for practical applications in nonvolatile memories. We showed that,during the forming and set processes, the compliance current, Icomp, can work as a crucial parameter to reduce IR. Doping with Co or Mn can significantly reduce the leakage current in capacitors made using SrTiOx film, opening a larger operation window for Icomp. By decreasing Icomp with acceptor doping, we could reduce IR in SrTiOx films by a factor of approximately 20. Our work suggests that the decrease of Icomp by carrier doping could be a viable alternative for reducing IR in unipolar resistance switching.",1003.1390v1 2011-11-01,High pressure transport properties of the topological insulator Bi2Se3,"We report x-ray diffraction, electrical resistivity, and magnetoresistance measurements on Bi2Se3 under high pressure and low temperature conditions. Pressure induces profound changes in both the room temperature value of the electrical resistivity as well as the temperature dependence of the resistivity. Initially, pressure drives Bi2Se3 towards increasingly insulating behavior and then, at higher pressures, the sample appears to enter a fully metallic state coincident with a change in the crystal structure. Within the low pressure phase, Bi2Se3 exhibits an unusual field dependence of the transverse magnetoresistance that is positive at low fields and becomes negative at higher fields. Our results demonstrate that pressures below 8 GPa provide a non-chemical means to controllably reduce the bulk conductivity of Bi2Se3.",1111.0098v1 2011-11-14,Study of Resistive Micromegas in a Mixed Neutron and Photon Radiation Field,"The Muon ATLAS Micromegas Activity (MAMMA) focuses on the development and testing of large-area muon detectors based on the bulk-Micromegas technology. These detectors are candidates for the upgrade of the ATLAS Muon System in view of the luminosity upgrade of Large Hadron Collider at CERN (sLHC). They will combine trigger and precision measurement capability in a single device. A novel protection scheme using resistive strips above the readout electrode has been developed. The response and sparking properties of resistive Micromegas detectors were successfully tested in a mixed (neutron and gamma) high radiation field supplied by the Tandem accelerator, at the N.C.S.R. Demokritos in Athens. Monte-Carlo studies have been employed to study the effect of 5.5 MeV neutrons impinging on Micromegas detectors. The response of the Micromegas detectors on the photons originating from the inevitable neutron inelastic scattering on the surrounding materials of the experimental facility was also studied.",1111.3185v1 2015-01-26,Linear magneto-resistance versus weak antilocalization effects in Bi$_2$Te$_3$ films,"In chalcogenide topological insulator materials, two types of magneto-resistance (MR) effects are widely discussed: a positive MR dip around zero magnetic field associated with the weak antilocalization (WAL) effect and a linear MR effect which generally persists to high fields and high temperatures. We have studied the MR of topological insulator Bi2Te3 films from the metallic to semiconducting transport regime. While in metallic samples, the WAL is difficult to identify due to the smallness of the WAL compared to the samples' conductivity, the sharp WAL dip in the MR is clearly present in the samples with higher resistivity. To correctly account for the low field MR by the quantitative theory of WAL according to the Hikami-Larkin-Nagaoka (HLN) model, we find that the classical (linear) MR effect should be separated from the WAL quantum correction. Otherwise the WAL fitting alone yields an unrealistically large coefficient $\alpha$ in the HLN analysis.",1501.06500v2 2018-04-05,Observation of transition from semiconducting to metallic ground state in high-quality single crystalline FeSi,"We report anomalous physical properties of single-crystalline FeSi over a wide temperature range 1.8-400 K. X-ray diffraction, specific heat, and magnetization measurements indicate that the FeSi crystals synthesized in this study are of high quality with a very low concentration of magnetic impurities ($\sim$0.01$\%$). The electrical resistivity $\rho$($T$) can be described by activated behavior with an energy gap $\Delta$ = 57 meV between 67 K and 150 K. At temperatures below 67 K, $\rho$($T$) is significantly lower than an extrapolation of the activated behavior, and the Hall coefficient and magneto-resistivity undergo a sign change in this region. At $\sim$19 K, a transition from semiconducting to metallic-like behavior is observed with deceasing temperature. Whereas the transition temperature is very robust in a magnetic field, the magnitude of the resistivity below $\sim$30 K is very sensitive to magnetic field. There is no indication of a bulk phase transition or onset of magnetic order in the vicinity of either 67 K or 19 K from specific heat and magnetic susceptibility measurements. These measurements provide evidence for a conducting surface state in FeSi at low temperatures.",1804.02036v1 2014-08-12,Nematic spin correlations in the tetragonal state of uniaxial strained BaFe2-xNixAs2,"Understanding the microscopic origins of electronic phases in high-transition temperature (high-Tc) superconductors is important for elucidating the mechanism of superconductivity. In the paramagnetic tetragonal phase of BaFe2-xTxAs2 (where T is Co or Ni) iron pnictides, an in-plane resistivity anisotropy has been observed. Here we use inelastic neutron scattering to show that low-energy spin excitations in these materials change from four-fold symmetric to two-fold symmetric at temperatures corresponding to the onset of the in-plane resistivity anisotropy. Because resistivity and spin excitation anisotropies both vanish near optimal superconductivity, we conclude that they are likely intimately connected.",1408.2756v1 2017-07-01,Memory vs. irreversibility in thermal densification of amorphous glasses,"We report on dynamic effects associated with thermally-annealing amorphous indium-oxide films. In this process the resistance of a given sample may decrease by several orders of magnitude at room-temperatures, while its amorphous structure is preserved. The main effect of the process is densification - increased system density. The study includes the evolution of the system resistivity during and after the thermal-treatment, the changes in the conductance-noise, and accompanying changes in the optical properties. The sample resistance is used to monitor the system dynamics during the annealing period as well as the relaxation that ensues after its termination. These reveal slow processes that fit well a stretched-exponential law, a behavior that is commonly observed in structural glasses. There is an intriguing similarity between these effects and those obtained in high-pressure densification experiments. Both protocols exhibit the ""slow spring-back"" effect, a familiar response of memory-foams. A heuristic picture based on a modified Lennard-Jones potential for the effective interparticle interaction is argued to qualitatively account for these densification-rarefaction phenomena in amorphous materials whether affected by thermal-treatment or by application of high-pressure.",1707.00173v1 2021-05-24,Characterization of self-heating in cryogenic high electron mobility transistors using Schottky thermometry,"Cryogenic low noise amplifiers based on high electron mobility transistors (HEMTs) are widely used in applications such as radio astronomy, deep space communications, and quantum computing, and the physical mechanisms governing the microwave noise figure are therefore of practical interest. In particular, the contribution of thermal noise from the gate at cryogenic temperatures remains unclear owing to a lack of experimental measurements of thermal resistance under these conditions. Here, we report measurements of gate junction temperature and thermal resistance in a HEMT at cryogenic and room temperatures using a Schottky thermometry method. At temperatures $\sim 20$ K, we observe a nonlinear trend of thermal resistance versus power that is consistent with heat dissipation by phonon radiation. Based on this finding, we consider heat transport by phonon radiation at the low-noise bias and liquid helium temperatures and estimate that the thermal noise from the gate is several times larger than previously assumed owing to self-heating. We conclude that without improvements in thermal management, self-heating results in a practical lower limit for microwave noise figure of HEMTs at cryogenic temperatures.",2105.11571v1 2021-10-06,Temperature dependent striction effect in a single crystalline Nd2Fe14B revealed using a novel high temperature resistivity measurement technique,"We studied the temperature dependence of resistivity in a single crystalline Nd2Fe14B using a newly developed high temperature probe. This novel probe uses mechanical pin connectors instead of conducting glue/paste. From warming and cooling curves, the Curie temperature was consistently measured around Tc = 580 K. In addition, anomalous discrete jumps were found only in cooling curves between 400 and 500 K, but not shown in warming curves. More interestingly, when the jumps occurred during cooling, the resistivity was increased. This phenomenon can be understood in terms of temperature dependent striction effect induced by the re-orientation of magnetic domains well below the Curie temperature.",2110.02909v1 2022-11-15,Pressure-Induced Insulator-to-Metal Transition in van der Waals compound CoPS$_3$,"We have studied the insulator-to-metal transition and crystal structure evolution under high pressure in the van der Waals compound CoPS$_3$ through $\textit{in-situ}$ electrical resistance, Hall resistance, magnetoresistance, X-ray diffraction, and Raman scattering measurements. CoPS$_3$ exhibits a $C2/m$ $\rightarrow$ $P\overline{3}$ structural transformation at 7 GPa accompanied by a 2.9$\%$ reduction in the volume per formula unit. Concomitantly, the electrical resistance decreases significantly, and CoPS$_3$ becomes metallic. This metallic CoPS$_3$ is a hole-dominant conductor with multiple conduction bands. The linear magnetoresistance and the small volume collapse at the metallization suggest the incomplete high-spin $\rightarrow$ low-spin transition in the metallic phase. Thus, the metallic CoPS$_3$ possibly possesses an inhomogeneous magnetic moment distribution and short-range magnetic ordering. This report summarizes the comprehensive phase diagram of $M$PS$_3$ ($M$ = V, Mn, Fe, Co, Ni, and Cd) that metalize under pressures.",2211.07925v4 2020-05-03,Resistive Switching Behaviour of Organic Molecules,"Organic electronics is very promising due to the flexibility, modifiability as well as variety of the available organic molecules. Efforts are going on to use organic materials for the realization of memory devices. In this regard resistive switching devices surely will play a key role. In this paper an effort has been made to illustrate the general information about resistive switching devices as well as switching mechanisms involving organic materials. As a whole a general overview of the emerging topic resistive switching has been given.",2005.01033v1 2023-06-17,An account of Natural material based Non Volatile Memory Device,"The development in electronic sector has brought a remarkable change in the life style of mankind. At the same time this technological advancement results adverse effect on environment due to the use of toxic and non degradable materials in various electronic devices. With the emergence of environmental problems, the green, reprogrammable, biodegradable, sustainable and environmental-friendly electronic devices have become one of the best solutions for protecting our environment from hazardous materials without compromising the growth of the electronic industry. Natural material has emerged as the promising candidate for the next generation electronic devices due to its easy processing, transparency, flexibility, abundant resources, sustainability, recyclability, and simple extraction. This review targets the characteristics, advancements, role, limitations, and prospects of using natural materials as the functional layer of a resistive switching memory device with a primary focus on the switching/memory properties. Among the available memory devices, resistive random access memory (RRAM), write once read many (WORM) unipolar memory etc. devices have a huge potential to become the non-volatile memory of the next generation owing to their simple structure, high scalability, and low power consumption. The motivation behind this work is to promote the use of natural materials in electronic devices and attract researchers towards a green solution of hazardous problems associated with the electronic devices.",2306.10382v1 2016-10-10,Determination of the resistivity anisotropy of orthorhombic materials via transverse resistivity measurements,"Measurements of the resistivity anisotropy can provide crucial information about the electronic structure and scattering processes in anisotropic and low-dimensional materials, but quantitative measurements by conventional means often suffer very significant systematic errors. Here we describe a novel approach to measuring the resistivity anisotropy of orthorhombic materials, using a single crystal and a single measurement, that is derived from a $\frac{\pi}{4}$ rotation of the measurement frame relative to the crystallographic axes. In this new basis the transverse resistivity gives a direct measurement of the resistivity anisotropy, which combined with the longitudinal resistivity also gives the in-plane elements of the conventional resistivity tensor via a 5-point contact geometry. This is demonstrated through application to the charge-density wave compound ErTe$_3$, and it is concluded that this method presents a significant improvement on existing techniques in many scenarios.",1610.03122v1 2019-08-28,Temperature-dependent hardness of diamond-structured covalent materials,"Understanding temperature-dependent hardness of covalent materials is not only of fundamental scientific interest, but also of crucial importance for technical applications. In this work, a temperature-dependent hardness formula for diamond-structured covalent materials is constructed on the basis of the dislocation theory. Our results show that, at low temperature, the Vickers hardness is mainly controlled by Poisson's ratio and shear modulus with the latter playing a dominant role. With increasing temperature, the plastic deformation mechanism undergoes a transition from shuffle-set dislocation control to glide-set dislocation control, leading to a steeper drop of hardness at high temperature. In addition, an intrinsic parameter, a3G, is revealed for diamond-structured covalent materials, which measures the resistance to soften at high temperature. Our hardness model shows remarkable agreement with experimental data. Current work not only sheds lights on the physical origin of hardness, but also provides a direct principle for superhard materials design.",1909.11032v2 2014-06-11,Evidence of surface transport and weak anti-localization in single crystal of Bi2Te2Se topological insulator,"Topological insulators are known to their metallic surface states, a result of strong-spin-orbital coupling, that show unique surface transport phenomenon. But these surface transports are buried in presence of metallic bulk conduction. We synthesized very high quality Bi$_2$Te$_2$Se single crystals by modified Bridgman method, that possess high bulk resistivity of $>$20~$\Omega$cm below 20~K, whereas the bulk is mostly inactive and surface transport dominates. Temperature dependence resistivity follows the activation law like a gap semiconductor in temperature range 20-300~K. We designed a special measurement geometry, which aims to extract the surface transport from the bulk. This special geometry is applied to measure the resistance and found that Bi$_2$Te$_2$Se single crystal exhibits a cross over from bulk to surface conduction at 20~K. Simultaneously, the material also shows strong evidence of weak anti-localization in magneto-transport due to the protection against scattering by conducting surface states. This novel simple geometry is an easy route to find the evidence of surface transport in topological insulators, which are the promising materials for future spintronic applications.",1406.2879v1 2019-05-29,Growth of metallic delafossite PdCoO2 by molecular beam epitaxy,"The Pd, and Pt based ABO2 delafossites are a unique class of layered, triangular oxides with 2D electronic structure and a large conductivity that rivals the noble metals. Here, we report successful growth of the metallic delafossite PdCoO2 by molecular beam epitaxy (MBE). The key challenge is controlling the oxidation of Pd in the MBE environment where phase-segregation is driven by the reduction of PdCoO2 to cobalt oxide and metallic palladium. This is overcome by combining low temperature (300 {\deg}C) atomic layer-by-layer MBE growth in the presence of reactive atomic oxygen with a post-growth high-temperature anneal. Thickness dependence (5-265 nm) reveals that in the thin regime (<75 nm), the resistivity scales inversely with thickness, likely dominated by surface scattering; for thicker films the resistivity approaches the values reported for the best bulk-crystals at room temperature, but the low temperature resistivity is limited by structural twins. This work shows that the combination of MBE growth and a post-growth anneal provides a route to creating high quality films in this interesting family of layered, triangular oxides.",1905.12549v2 2019-06-21,Current localisation and redistribution as the basis of discontinuous current controlled negative differential resistance in NbOx,"In-situ thermo-reflectance imaging is used to show that the discontinuous, snap-back mode of current-controlled negative differential resistance (CC-NDR) in NbOx-based devices is a direct consequence of current localization and redistribution. Current localisation is shown to result from the creation of a conductive filament either during electroforming or from current bifurcation due to the super-linear temperature dependence of the film conductivity. The snap-back response then arises from current redistribution between regions of low and high current-density due to the rapid increase in conductivity created within the high current density region. This redistribution is further shown to depend on the relative resistance of the low current-density region with the characteristics of NbOx cross-point devices transitioning between continuous and discontinuous snap-back modes at critical values of film conductivity, area, thickness and temperature, as predicted. These results clearly demonstrate that snap-back is a generic response that arises from current localization and redistribution within the oxide film rather than a material-specific phase transition, thus resolving a long-standing controversy.",1906.08980v2 2017-12-03,Spin transport in two-layer-CVD-hBN/graphene/hBN heterostructures,"We study room temperature spin transport in graphene devices encapsulated between a layer-by-layer-stacked two-layer-thick chemical vapour deposition (CVD) grown hexagonal boron nitride (hBN) tunnel barrier, and a few-layer-thick exfoliated-hBN substrate. We find mobilities and spin-relaxation times comparable to that of SiO$_2$ substrate based graphene devices, and obtain a similar order of magnitude of spin relaxation rates for both the Elliott-Yafet and D'Yakonov-Perel' mechanisms. The behaviour of ferromagnet/two-layer-CVD-hBN/graphene/hBN contacts ranges from transparent to tunneling due to inhomogeneities in the CVD-hBN barriers. Surprisingly, we find both positive and negative spin polarizations for high-resistance two-layer-CVD-hBN barrier contacts with respect to the low-resistance contacts. Furthermore, we find that the differential spin injection polarization of the high-resistance contacts can be modulated by DC bias from -0.3 V to +0.3 V with no change in its sign, while its magnitude increases at higher negative bias. These features mark a distinctive spin injection nature of the two-layer-CVD-hBN compared to the bilayer-exfoliated-hBN tunnel barriers.",1712.00815v1 2004-09-06,"Calculation of resistance for weak scattering, strong scattering and insulating quasi-one dimensional systems","A parameter free calculation of the resistivity is applied to liquid metals near the melting point ranging from weak to strong scattering limit. The method is based on length dependent resistance calculations for quasi-one dimensional systems and was applied on structures with up to 10000 atoms. The calculated value for conductance fluctuations is in good agreement with theoretical predictions. The resistivities are compared with the Kubo-Greenwood and the extended Ziman formula with the same scattering potential and similar structure. The resistance calculation is applicable for insulating materials as well, which is demonstrated for crystalline and amorphous silicon.",0409131v2 2012-07-02,Magneto-resistance in three-dimensional composites,"In this paper we study the magneto-resistance, i.e. the second-order term of the resistivity perturbed by a low magnetic field, of a three-dimensional composite material. Extending the two-dimensional periodic framework of [4], it is proved through a H-convergence approach that the dissipation energy induced by the effective magneto-resistance is greater or equal to the average of the dissipation energy induced by the magneto-resistance in each phase of the composite. This inequality validates for a composite material the Kohler law which is known for a homogeneous conductor. The case of equality is shown to be very sensitive to the magnetic fi eld orientation. We illustrate the result with layered and columnar periodic structures.",1207.0468v1 2020-06-30,Roadmap for Gain-Bandwidth-Product Enhanced Photodetectors,"Photodetectors are key optoelectronic building blocks performing the essential optical-to-electrical signal conversion, and unlike solar cells, operate at a specific wavelength and at high signal or sensory speeds. Towards achieving high detector performance, device physics, however, places a fundamental limit of the achievable detector sensitivity, such as responsivity and gain, when simultaneously aimed to increasing the detectors temporal response, speed, known as the gain-bandwidth product (GBP). While detectors GBP has been increasing in recent years, the average GBP is still relatively modest (~10^6-10^7 Hz-A/W). Here we discuss photodetector performance limits and opportunities based on arguments from scaling length theory relating photocarrier channel length, mobility, electrical resistance with optical waveguide mode constrains. We show that short-channel detectors are synergistic with slot-waveguide approaches, and when combined, offer a high-degree of detector design synergy especially for the class of nanometer-thin materials. Indeed, we find that two dimensional material-based detectors are not limited by their low mobility and can, in principle, allow for 100 GHz fast response rates. However, contact resistance is still a challenge for such thin materials, a research topic that is still not addressed yet. An interim solution is to utilize heterojunction approaches for functionality separation. Nonetheless, atomistically- and nanometer-thin materials used in such next-generation scaling length theory based detectors also demand high material quality and monolithic integration strategies into photonic circuits including foundry-near processes. As it stands, this letter aims to guide the community if achieving the next generation photodetectors aiming for a performance target of GBP = 10^12 Hz-A/W.",2006.16937v1 2005-06-01,Insulator-metal transition in a conservative system: An evidence for mobility coalescence in island silver films,"Aging, which manifests itself as an irreversible increase in electrical resistance in island metal films is of considerable interest from both academic as well as applications point of view. Aging is attributed to various causes, oxidation of islands and mobility of islands followed by coalescence (mobility coalescence) being the main contenders. The effect of parameters like substrate temperature, substrate cleaning, residual gases in the vacuum chamber, ultrasonic vibration of the substrate, suggest that the mobility coalescence is responsible for the aging in island metal films. Electron microscopy studies show evidence for mobility of islands at high substrate temperatures. The comparison of aging data of island silver films deposited on glass substrates in ultra high vacuum and high vacuum suggests that the oxidation of islands, as being responsible for aging in these films, can be ruled out. Further, under certain conditions of deposition, island silver films exhibit a dramatic and drastic fall in electrical resistance, marking the insulator-metal transition. This interesting transition observed in a conservative system - after the stoppage of deposition of the film- is a clear evidence for mobility coalescence of islands even at room temperature. The sudden fall in resistance is preceded by fluctuations in resistance with time and fluctuations are attributed to the making and breaking of the percolation path in the film.",0506022v2 2010-09-22,Hall-effect and resistivity measurements in CdTe and ZnTe at high pressure: Electronic structure of impurities in the zincblende phase and the semi-metallic or metallic character of the high-pressure phases,"We carried out high-pressure resistivity and Hall-effect measurements in single crystals of CdTe and ZnTe up to 12 GPa. Slight changes of transport parameters in the zincblende phase of CdTe are consitent with the shallow character of donor impurities. Drastic changes in all the transport parameters of CdTe were found around 4 GPa, i.e. close to the onset of the cinnabar to rock-salt transition. In particular, the carrier concentration increases by more than five orders of magnitude. Additionally, an abrupt decrease of the resistivity was detected around 10 GPa. These results are discussed in comparison with optical, thermoelectric, and x-ray diffraction experiments. The metallic character of the Cmcm phase of CdTe is confirmed and a semi-metallic character is determined for the rock-salt phase. In zincblende ZnTe, the increase of the hole concentration by more than two orders of magnitude is proposed to be due to a deep-to-shallow transformation of the acceptor levels. Between 9 and 11 GPa, transport parameters are consistent with the semiconducting character of cinnabar ZnTe. A two orders of magnitude decrease of the resistivity and a carrier-type inversion occurs at 11 GPa, in agreement with the onset of the transition to the Cmcm phase of ZnTe. A metallic character for this phase is deduced.",1009.4304v1 2019-10-18,Atomically Controlled Tunable Doping in High Performance WSe2 Devices,"Two-dimensional transitional metal dichalcogenide (TMD) field-effect transistors (FETs) are promising candidates for future electronic applications, owing to their excellent transport properties and potential for ultimate device scaling. However, it is widely acknowledged that substantial contact resistance associated with the contact-TMD interface has impeded device performance to a large extent. It has been discovered that O2 plasma treatment can convert WSe2 into WO3-x and substantially improve contact resistances of p-type WSe2 devices by strong doping induced thinner depletion width. In this paper, we carefully study the temperature dependence of this conversion, demonstrating an oxidation process with a precise monolayer control at room temperature and multilayer conversion at elevated temperatures. Furthermore, the lateral oxidation of WSe2 under the contact revealed by HR-STEM leads to potential unpinning of the metal Fermi level and Schottky barrier lowering, resulting in lower contact resistances. The p-doping effect is attributed to the high electron affinity of the formed WO3-x layer on top of the remaining WSe2 channel, and the doping level is found to be dependent on the WO3-x thickness that is controlled by the temperature. Comprehensive materials and electrical characterizations are presented, with a low contact resistance of ~528 ohm-um and record high on-state current of 320 uA/um at -1V bias being reported.",1910.08619v1 2004-03-23,Systematic approach to the growth of high-quality single-crystals of Sr3Ru2O7,"We describe a simple procedure for optimising the growth condition for high quality single crystals of the strontium ruthenate perovskites using an image furnace. The procedure involves carefully measuring the mass lost during crystal growth in order to predict the optimal initial atomic ratio. Using this approach we have succeeded in growing crystals of Sr3Ru2O7 with a residual resistivity as low as 0.25 ??cm. The procedure we describe here is expected to be useful for other systems when a standard travelling-solvent floating-zone (TSFZ) method cannot be used because of high volatility of a constituent material.",0403572v1 2022-03-22,High-field magnetoresistance of microcrystalline and nanocrystalline Ni metal at 3 K and 300 K,"The magnetoresistance (MR) and the magnetization isotherms were studied up to high magnetic fields at T = 3 K and 300 K for a microcrystalline ($\mu$c) Ni foil corresponding to bulk Ni and for a nanocrystalline (nc) Ni foil. At T = 3 K, for the $\mu$c-Ni sample with a residual resistivity ratio (RRR) of 331, the field dependence of the resistivity was similar to what was reported previously for high-purity ferromagnets whereas the MR(H) behavior for the nc-Ni sample with RRR = 9 resembled that what was observed at low temperatures for Ni-based alloys with low impurity concentration. In the magnetically saturated state, the resistivity increased with magnetic field for both samples at T = 3 K and the field dependence was dominated by the ordinary MR due to the Lorentz force acting on the electron trajectories. However, the MR(H) curves were found to be saturating for $\mu$c-Ni and non-saturating for nc-Ni, the difference arising from their very different electron mean free paths. At T = 300 K, the MR(H) curves of both Ni samples were very similar to those known for bulk Ni. After magnetic saturation, the resistivity decreased nearly linearly with magnetic field which behavior is due to the suppression of thermally-induced magnetic disorder with increasing magnetic field. The MR(H) data were analyzed at both temperatures with the help of Kohler plots from which the resistivity anisotropy splitting ($\Delta\rho_{AMR}$) and the anisotropic magnetoresistance (AMR) ratio were derived. It was demonstrated that at T = 300 K, $\rho(H\rightarrow 0)=\rho(B\rightarrow 0)$ due to the negligible contribution of the ordinary MR. The data for the two Ni samples at 3 K and 300 K were found to indicate an approximately linear scaling of $\Delta\rho_{AMR}$ with the zero-field resistivity. This implies that the AMR ratio does not vary significantly with temperature in either microstructural state of Ni.",2203.11568v1 2023-09-18,Theoretical analysis on the possibility of superconductivity in a trilayer Ruddlesden-Popper nickelate La$_4$Ni$_3$O$_{10}$ under pressure and its experimental examination: comparison with La$_3$Ni$_2$O$_7$,"We study the possibility of superconductivity in a trilayer Ruddlesden-Popper nickelate La$_4$Ni$_3$O$_{10}$ under pressure both theoretically and experimentally, making comparison with the recently discovered high $T_c$ superconductor La$_3$Ni$_2$O$_7$, a bilayer nickelate. Through DFT calculations, we find that a structural phase transition from monoclinic to tetragonal takes place around 10 - 15 GPa. Using the tetragonal crystal structure, we theoretically investigate the possibility of superconductivity, where a combination of fluctuation exchange approximation and linearized Eliashberg equation is applied to a six-orbital model constructed from first principles band calculation. The obtained results suggests that La$_4$Ni$_3$O$_{10}$ may also become superconducting under high pressure with $T_c$ comparable to some cuprates, although it is not as high as La$_3$Ni$_2$O$_7$. We also perform experimental studies using our polycrystalline samples of La$_3$Ni$_2$O$_{7.01}$ and La$_4$Ni$_3$O$_{9.99}$. The superconducting transition of La$_3$Ni$_2$O$_{7.01}$, with a maximum onset $T_c$ of 67.0 K at a pressure of 26.5 GPa, is confirmed by a drop in the electrical resistance, as well as the magnetic field dependence of the resistance. Quite interestingly, similar temperature and magnetic field dependencies of the resistance are observed also for La$_4$Ni$_3$O$_{9.99}$, where a drop in the resistance is observed at lower temperatures compared to La$_3$Ni$_2$O$_{7.01}$, under pressures of 32.8 GPa and above. Given the theoretical expectation, the reduction in the resistance can most likely be attributed to the occurrence of superconductivity in La$_4$Ni$_3$O$_{9.99}$. The temperature at which the resistance deviates from a linear behavior, considered as the onset $T_c$, monotonically increases up to 23 K at 79.2 GPa, which is opposite to the pressure dependence of $T_c$ in La3Ni2O7.01.",2309.09462v4 2019-07-16,"Pressure-Induced Large Volume Collapse, Plane-to-Chain, Insulator to Metal Transition in CaMn$_2$Bi$_2$","In-situ high pressure single crystal X-ray diffraction study reveals that the quantum material CaMn$_2$Bi$_2$ undergoes a unique plane to chain structural transition between 2 and 3 GPa, accompanied by a large volume collapse. CaMn2Bi2 displays a new structure type above 2.3 GPa, with the puckered Mn honeycomb lattice of the trigonal ambient-pressure structure converting to one-dimensional (1D) zigzag chains in the high-pressure monoclinic structure. Single crystal measurements reveal that the pressure-induced structural transformation is accompanied by a dramatic two order of magnitude drop of resistivity; although the ambient pressure phase displays semiconducting behavior at low temperatures, metallic temperature dependent resistivity is observed for the high pressure phase, as, surprisingly, are two resistivity anomalies with opposite pressure dependences. Based on the electronic structure calculations, we hypothesized that the newly emerged electronic state under high pressure is associated with a Fermi surface instability of the quasi-1D Mn chains, while we infer that the other is a magnetic transition. Assessment of the total energies for hypothetical magnetic structures for high pressure CaMn$_2$Bi$_2$ indicates that ferrimagnetism is thermodynamically favored.",1907.07203v1 2014-10-09,Chloride Molecular Doping Technique on 2D Materials: WS2 and MoS2,"Low-resistivity metal-semiconductor (M-S) contact is one of the urgent challenges in the research of 2D transition metal dichalcogenides (TMDs). Here, we report a chloride molecular doping technique which greatly reduces the contact resistance (Rc) in the few-layer WS2 and MoS2. After doping, the Rc of WS2 and MoS2 have been decreased to 0.7 kohm*um and 0.5 kohm*um, respectively. The significant reduction of the Rc is attributed to the achieved high electron doping density thus significant reduction of Schottky barrier width. As a proof-ofconcept, high-performance few-layer WS2 field-effect transistors (FETs) are demonstrated, exhibiting a high drain current of 380 uA/um, an on/off ratio of 4*106, and a peak field-effect mobility of 60 cm2/V*s. This doping technique provides a highly viable route to diminish the Rc in TMDs, paving the way for high-performance 2D nano-electronic devices.",1410.2563v1 2021-04-08,Electrical Properties of Selective-Area-Grown Superconductor-Semiconductor Hybrid Structures on Silicon,"We present a superconductor-semiconductor material system that is both scalable and monolithically integrated on a silicon substrate. It uses selective area growth of Al-InAs hybrid structures on a planar III-V buffer layer, grown directly on a high resistivity silicon substrate. We characterized the electrical properties of this material system at millikelvin temperatures and observed a high average field-effect mobility of $\mu \approx 3200\,\mathrm{cm^2/Vs}$ for the InAs channel, and a hard induced superconducting gap. Josephson junctions exhibited a high interface transmission, $\mathcal{T} \approx 0.75 $, gate voltage tunable switching current with a product of critical current and normal state resistance, $I_{\mathrm{C}}R_{\mathrm{N}} \approx 83\,\mathrm{\mu V}$, and signatures of multiple Andreev reflections. These results pave the way for scalable and high coherent gate voltage tunable transmon devices and other superconductor-semiconductor hybrids fabricated directly on silicon.",2104.03621v1 2021-09-21,Strain effects on the wear rate of severely deformed copper,"A variety of severe plastic deformation (SPD) techniques have been developed to process materials to high strains and impart microstructural refinement. High pressure torsion (HPT) is one technique that imparts inhomogeneous strain to process discs with low strain in the center and high strain at the outer edge. In the literature, this inhomogeneity is typically ignored when characterizing wear properties after HPT. In this work, the wear rate of pure copper discs processed by HPT was characterized by conducting dry sliding reciprocating wear tests at a few judicious locations on the discs. From only two discs, the wear resistance across many ranges of strains was captured. These measurements agreed with the literature for other SPD processes at varying strains. Wear rates dropped and plateaued at about 25% that of the unprocessed state when processing past equivalent strains of around 15, after which microstructural and microhardness saturation has also been observed. Some indication of a relationship between the direction of the imposed SPD shearing and the sliding wear direction was also observed. The incremental microstructure, microhardness, and wear resistance evolution past equivalent strains of ~15 indicate that for high purity copper these properties receive no clear benefit from higher SPD strains.",2109.09907v1 2016-07-07,Lithium transport through Lithium-ion battery cathode coatings,"The surface coating of cathodes using insulator films has proven to be a promising method for high-voltage cathode stabilization in Li-ion batteries. However, there is still substantial uncertainty about how these films function, specifically with regard to important coating design principles such as lithium solubility and transport through the films. This study uses Density Functional Theory to examine the diffusivity of interstitial lithium in crystalline {\alpha}-$AlF_3$, {\alpha}-$Al_2O_3$, m-$ZrO_2$, c-MgO, and {\alpha}-quartz $SiO_2$, which provide benchmark cases for further understanding of insulator coatings in general. In addition, we propose an Ohmic electrolyte model to predict resistivities and overpotential contributions under battery operating conditions. For the crystalline materials considered we predict that Li+ diffuses quite slowly, with a migration barrier larger than 0.9 eV in all crystalline materials except {\alpha}-quartz $SiO_2$, which is predicted to have a migration barrier of 0.276 eV along <001>. These results suggest that the stable crystalline forms of these insulator materials, except for oriented {\alpha}-quartz $SiO_2$, are not practical for conformal cathode coatings. Amorphous $Al_2O_3$ and $AlF_3$ have higher Li+ diffusivities than their crystalline counterparts. Our predicted amorphous $Al_2O_3$ resistivity (1789 M{\Omega}m) is near the top of the range of fitted resistivities extracted from previous experiments on nominal $Al_2O_3$ coatings (7.8 to 913 M{\Omega}m) while our predicted amorphous $AlF_3$ resistivity (114 M{\Omega}m) is close to the middle of the range. These comparisons support our framework for modeling and understanding the impact on overpotential of conformal coatings in terms of their fundamental thermodynamic and kinetic properties, and support that these materials can provide practical conformal coatings in their amorphous form.",1607.02125v1 2023-04-20,An Origami-Inspired Design of Highly Efficient Cellular Cushion Materials,"Current architectured cellular cushion materials rely mainly on damage and/or unpredictable collapse of their unit cells to absorb and dissipate energy under impact. This prevents shape recovery and produces undesirable force fluctuations that limit reusability and reduce energy absorption efficiency. Here, we propose to combine advanced manufacturing technologies with Origami principles to create a new class of architectured cellular viscoelastic cushion material which combines low weight and high energy absorption efficiency with damage resistance and full behavior customization. Each unit cell in the proposed material is inspired by the Kresling Origami topology, which absorbs impact energy by gracefully folding the different interfaces forming the cell to create axial and rotational motions. A large part of the absorbed energy is then dissipated through viscoelasticity and friction between the interfaces. The result is a nearly ideal cushion material exhibiting high energy absorbing efficiency (around 70%) combined with high energy dissipation (94% of the absorbed energy). The material is also tunable for optimal performance, reliable despite successive impact events, and achieves full shape recovery.",2304.10238v1 2024-01-28,"Discharge quenching mechanism and performance of RPWELL with tunable 3D printed resistive plates, charge evacuation in semiconductive glass RPWELL and discharge quenching for Cryogenic-RWELL over a wide range of resistivity","Resistive electrodes are used in gaseous detectors to quench electrical discharges. This helps to protect delicate electrodes and readout electronics and to improve the stability of the detector operation. An RPWELL is a THGEM-based WELL detector with a resistive plate coupled to a conductive anode. Till now, the choice of the resistive plate was limited to a few materials, like LRS Glass and Semitron. These materials have fixed resistivities and, sometimes, thickness and area limitations. This restricts the potential usage of the detector to a rather small range of applications, as well as the possibility of studying in depth the physics processes governing the discharge quenching mechanism. In our present study, we used a new plastic material doped with carbon nanotubes to produce resistive plates with a commercial 3D printer. This method has the flexibility to produce samples of different thicknesses and different resistivity values. We describe here the sample production and characterize the RPWELL performance with different resistive plates. In particular we show the dependence of discharge quenching on the thickness and resistivity of the plate. The dynamics of the charge carriers in the material is proposed as an explanation for the long gain recovery time after a discharge.",2401.15611v2 2009-09-25,Electric field-induced colossal electroresistance and its relaxation in multiferroic La2NiMnO6,"In this work, we report direct as well as pulsed electric field-induced resistivity switching and its relaxation in a multiferroic insulator La2NiMnO6. At a fixed base temperature (Tb), the dc resistivity switches abruptly from a high to a low value, which is manifested as an upward jump in the dc current density (J) when the electric field (E) exceeds a threshold value Eth. The fractional change in the resistance is as much as 70 % at room temperature for Eth = 95 V/cm. The Eth increases with lowering Tb and follows the relation Eth(Tb) = Eth(0)exp[-Tb/T0], as similar to the behavior found in charge density wave systems. It is shown that the abrupt jump in J vanishes under pulsed electric fields if the period between pulses is long enough. Surprisingly, a step-like increase in J also occurs at a fixed dc electric field (Ec) and T = Tb, above a threshold waiting time (tth). The tth decreases with increasing Ec and Tb. Simultaneous measurement of surface temperature during the J-E sweep and temporal studies suggest that conductive channels are created in an insulating matrix due to the local self heating, and the coalescence of these channels above a threshold E- field or time causes the observed anomalies in J. However, the dissipated Joule power (P = Ith2R) at the transition from high to low resistive state in the sample decreases with lowering temperature, which suggests that the Joule heating is the consequence of transition from the high to low resistance state rather than itself a driving force of the non linear electrical transport. In addition, non linear J-E characteristics is also found even with a pulsed voltage sweep, which suggests that intrinsic mechanisms other than self heating is still active in this material.",0909.4612v1 2022-07-10,"Diffusion theory of electrical contact resistance of ""thermoelectric superlattice metal"" couple","The paper proposes a strict diffusion theory of the electrical contact resistance of a thermoelectric superlattice (TES) - metal couple.The limits of the contact resistance for traditional thermoeletric materials with parabolic band spectrum and for superlattices described by Fivaz model are estimated.",2207.05065v1 2018-01-30,Open Material Property Library With Native Simulation Tool Integrations -- MASTO,"Reliable material property data is crucial for trustworthy simulations throughout different areas of engineering. Special care must be taken when materials at extreme conditions are under study. Superconductors and devices assembled from superconductors and other materials, like superconducting magnets, are often operated at such extreme conditions: at low temperatures under high magnetic fields and stresses. Typically, some library or database is used for getting the data. We have started to develop a database for storing all kind of material property data online called Open Material Property Library With Native Simulation Tool Integrations -- MASTO. The data that can be imported includes, but is not limited to, anisotropic critical current surfaces for high temperature superconducting materials, electrical resistivities as a function of temperature, RRR and magnetic field, general fits for describing material behaviour etc. Data can also depend on other data and it can be versioned to guarantee permanent access. The guiding idea in MASTO is to build easy-to-use integration for various programming languages, modelling frameworks and simulation software. Currently, a full-fledged integration is built for MATLAB to allow users to fetch and use data with one-liners. In this paper we briefly review some of the material property databases commonly used in superconductor modelling, present a case study showing how selection of the material property data can influence the simulation results, and introduce the principal ideas behind MASTO. This work serves as the reference document for citing MASTO when it is used in simulations.",1801.09897v1 2018-11-22,Chemical vapor deposition of hexagonal boron nitride and its use in electronic devices,"Dielectrics are insulating materials used in many different electronic devices and play an important role in all of them. Current advanced electronic devices use dielectric materials with a high dielectric constant and avoid high leakage currents. However, these materials show several intrinsic problems, and also a bad interaction with adjacent materials. Therefore, the race for finding a suitable dielectric material for current and future electronic devices is still open. In this context two dimensional [2D] materials have become a serious option, not only thanks to their advanced properties, but also to the development of scalable synthesis methods. Graphene has been the most explored 2D material for electronic devices. However, graphene has no band gap, and therefore it cannot be used as dielectric. MoS2 and other 2D transition metal dichalcogenides (TMDs) are semiconducting 2D materials that can provide more versatility in electronic devices. In this PhD thesis I have investigated the use of monolayer and multilayer hexagonal boron nitride (h-BN) as dielectric for electronic devices, as it is a 2D material with a band gap of ~5.9 eV. My work has mainly focused on the synthesis of the h-BN using chemical vapor deposition, the study of its intrinsic morphological and electrical properties at the nanoscale, and its performance as dielectric in different electronic devices, such as capacitors and memristors. Overall, our experiments indicate that h-BN is a very reliable dielectric material, and that it can be successfully used in capacitors and memristors. Moreover, h-BN shows additional performances never observed in traditional dielectrics, such as volatile resistive switching, which may also open the door for new applications.",1905.06938v1 2020-04-14,Materials Requirements of High-Speed and Low-Power Spin-Orbit-Torque Magnetic Random-Access Memory,"As spin-orbit-torque magnetic random-access memory (SOT-MRAM) is gathering great interest as the next-generation low-power and high-speed on-chip cache memory applications, it is critical to analyze the magnetic tunnel junction (MTJ) properties needed to achieve sub-ns, and ~fJ write operation when integrated with CMOS access transistors. In this paper, a 2T-1MTJ cell-level modeling framework for in-plane type Y SOT-MRAM suggests that high spin Hall conductivity and moderate SOT material sheet resistance are preferred. We benchmark write energy and speed performances of type Y SOT cells based on various SOT materials experimentally reported in the literature, including heavy metals, topological insulators and semimetals. We then carry out detailed benchmarking of SOT material Pt, beta-W, and BixSe(1-x) with different thickness and resistivity. We further discuss how our 2T-1MTJ model can be expanded to analyze other variations of SOT-MRAM, including perpendicular (type Z) and type X SOT-MRAM, two-terminal SOT-MRAM, as well as spin-transfer-torque (STT) and voltage-controlled magnetic anisotropy (VCMA)-assisted SOT-MRAM. This work will provide essential guidelines for SOT-MRAM materials, devices, and circuits research in the future.",2004.06268v2 2022-04-28,Degradation model of high-nickel positive electrodes: Effects of loss of active material and cyclable lithium on capacity fade,"Nickel-rich layered oxides have been widely used as positive electrode materials for high-energy-density lithium-ion batteries, but their degradation has severely affected cell performance, in particular at a high voltage and temperature. However, the underlying degradation mechanisms have not been well understood due to the complexity and lack of predictive models.Here we present a model at the particle level to describe the structural degradation caused by phase transition in terms of loss of active material (LAM), loss of lithium inventory (LLI), and resistance increase. The particle degradation model is then incorporated into a cell-level P2D model to explore the effects of LAM and LLI on capacity fade in cyclic ageing tests. It is predicted that the loss of cyclable lithium (trapped in the degraded shell) leads to a shift in the stoichiometry range of the negative electrode but does not directly contribute to the capacity loss, and that the loss of positive electrode active materials dominates the fade of usable cell capacity in discharge. The available capacity at a given current rate is further decreased by the additional resistance of the degraded shell layer. The change pattern of the state-of-charge curve provides information of more dimensions than the conventional capacity-fade curve, beneficial to the diagnosis of degradation modes. The model has been implemented into PyBaMM and made available as open source codes.",2204.13364v2 2019-02-26,Data-driven Exploration of Pressure-Induced Superconductivity in AgIn$_{5}$Se$_{8}$,"Candidates compounds for new thermoelectric and superconducting materials, which have narrow band gap and flat bands near band edges, were exhaustively searched by a high-throughput first-principles calculation from an inorganic materials database named AtomWork. We focused on AgIn$_{5}$Se$_{8}$ which has high density of state near the Fermi level. AgIn$_{5}$Se$_{8}$ was successfully synthesized as single crystals using a melt and slow cooling method. The single-crystal X-ray diffraction analysis revealed the obtained crystal is high quality without deficiencies. The valence states in AgIn$_{5}$Se$_{8}$ were determined to be Ag1+, In3+ and Se2- in accordance with a formal charge by the core level X-ray photoelectron spectroscopy analysis. The electrical resistance was evaluated under high pressure using a diamond anvil cell with boron-doped diamond electrodes. Although the sample was insulator with a resistance of above 40 M{\Omega} at ambient pressure, the resistance markedly decreased with increase of the pressure, and a pressure-induced superconducting transition was discovered at 3.4 K under 52.5 GPa. The transition temperature increased up to 3.7 K under further pressure of 74.0 GPa.",1902.09770v1 2020-06-25,"Influence of Yb3+on the structural, electrical and optical properties of sol-gel synthesized Ni-Zn nanoferrites","Polycrystalline Yb substituted NiZn nanoferrites with the compositions of Ni0.5Zn0.5YbxFe2-xO4 (x= 0.00, 0.04, 0.08, 0.12, 0.16 and 0.20) have been synthesized using sol gel auto combustion technique. Single phase cubic spinel structure has been confirmed by the X ray diffraction (XRD) patterns. Larger lattice constants of the compositions are found with increasing Yb3+ concentration while the average grain size (52 to 18 nm) has noticeable decrease as Yb3+ content is increased. The presence of all existing elements as well as the purity of the samples has also been confirmed from energy dispersive X ray spectroscopic (EDS) analysis. Frequency dependent dielectric constant, dielectric loss, dielectric relaxation time, AC and DC resistivity of the compositions have also been examined at room temperature. The DC resistivity value is found in the order of 10 to power 10 (omega-cm) which is at least four orders greater than the ferrites prepared by conventional method. This larger value of resistivity attributes due to very small grain size and successfully explained using the Verwey and deBoer hopping conduction model. The contribution of grain and grain boundary resistance has been elucidated using Cole Cole plot. The study of temperature dependent DC resistivity confirms the semiconducting nature of all titled compositions wherein bandgap (optical) increases from 2.73 eV to 3.25 eV with the increase of Yb content. The high value of resistivity is of notable achievement for the compositions that make them a potential candidate for implication in the high frequency applications where reduction of eddy current loss is highly required.",2006.14180v1 2024-04-12,"Electron-phonon interaction, magnetic phase transition, charge density waves and resistive switching in VS2 and VSe2 revealed by Yanson point contact spectroscopy","VS2 and VSe2 have attracted particular attention among the transition metals dichalcogenides because of their promising physical properties concerning magnetic ordering, charge density wave (CDW), emergent superconductivity, etc., which are very sensitive to stoichiometry and dimensionality reduction. Yanson point contact (PC) spectroscopic study reveals metallic and nonmetallic states in VS2 PCs, as well as a magnetic phase transition was detected below 25 K. Analysis of PC spectra of VS2 testifies the realization of the thermal regime in PCs. At the same time, rare PC spectra, where the magnetic phase transition was not visible, shows a broad maximum of around 20 mV, likely connected with electron-phonon interaction (EPI). On the other hand, PC spectra of VSe2 demonstrate metallic behavior, which allowed us to detect features associated with EPI and CDW transition. The Kondo effect appeared for both compounds, apparently due to interlayer vanadium ions. Besides, the resistive switching was observed in PCs on VSe2 between a low resistive, mainly metallic-type state, and a high resistive nonmetallic-type state by applying bias voltage (about 0.4V). In contrast, reverse switching occurs by applying a voltage of opposite polarity (about 0.4V). The reason may be the alteration of stoichiometry in the PC core due to the displacement of V ions to interlayer under a high electric field. The observed resistive switching characterize VSe2 as a potential material, e.g., for non-volatile resistive RAM, neuromorphic engineering, and for other nanoelectronic applications. At the same time, VSe2 attracts attention as a rare layered van der Waals compound with magnetic transition.",2404.08269v1 2010-11-12,Large bulk resistivity and surface quantum oscillations in the topological insulator Bi2Te2Se,"Topological insulators are predicted to present novel surface transport phenomena, but their experimental studies have been hindered by a metallic bulk conduction that overwhelms the surface transport. We show that a new topological insulator, Bi2Te2Se, presents a high resistivity exceeding 1 Ohm-cm and a variable-range hopping behavior, and yet presents Shubnikov-de Haas oscillations coming from the surface Dirac fermions. Furthermore, we have been able to clarify both the bulk and surface transport channels, establishing a comprehensive understanding of the transport in this material. Our results demonstrate that Bi2Te2Se is the best material to date for studying the surface quantum transport in a topological insulator.",1011.2846v1 2017-02-14,Modelling electron-phonon interactions in graphene with curved space hydrodynamics,"We introduce a different perspective describing electron-phonon interactions in graphene based on curved space hydrodynamics. Interactions of phonons with charge carriers increase the electrical resistivity of the material. Our approach captures the lattice vibrations as curvature changes in the space through which electrons move following hydrodynamic equations. In this picture, inertial corrections to the electronic flow arise naturally effectively producing electron-phonon interactions. The strength of the interaction is controlled by a coupling constant, which is temperature independent. We apply this model to graphene and recover satisfactorily the linear scaling law for the resistivity that is expected at high temperatures. Our findings open up a new perspective of treating electron-phonon interactions in graphene, and also in other materials where electrons can be described by the Fermi liquid theory.",1702.04156v1 2019-10-31,Vorticity of viscous electronic flow in graphene,"In ultra-pure materials electrons may exhibit a collective motion similar to the hydrodynamic flow of a viscous fluid, the phenomenon with far reaching consequences in a wide range of many body systems from black holes to high-temperature superconductivity. Yet the definitive detection of this intriguing behavior remains elusive. Until recently, experimental techniques for observing hydrodynamic behavior in solids were based on measuring macroscopic transport properties, such as the ""nonlocal"" (or ""vicinity"") resistance, which may allow alternative interpretation. Earlier this year two breakthrough experiments demonstrated two distinct imaging techniques making it possible to ""observe"" the electronic flow directly. We demonstrate that a hydrodynamic flow in a long Hall bar (in the absence of magnetic field) exhibits a nontrivial vortex structure accompanied by a sign-alternating nonlocal resistance. An experimental observation of such unique flow pattern could serve a definitive proof of electronic hydrodynamics.",1910.14473v2 2021-11-09,Magnetotransport in ferromagnetic Fe$_2$Ge semimetallic thin films,"Thin films of the ferromagnet Fe$_2$Ge were grown via molecular beam epitaxy, and their electrical and magneto-transport properties measured for the first time. X-ray diffraction and vibrating sample magnetometry measurements confirmed the crystalline ferromagnetic Fe$_2$Ge phase. The observed high temperature maximum in the longitudinal resistivity, as well as the observed suppression of electron-magnon scattering at low temperatures, point to the presence of strong spin polarization in this material. Measurements of the Hall resistivity, $\rho_{xy}$, show contributions from both the ordinary Hall effect and anomalous Hall effect, $\rho_{xy}^{AH}$, from which we determined the charge carrier concentration and mobility. Measurements also show a small negative magnetoresistance in both the longitudinal and transverse geometries. Fe$_2$Ge holds promise as a useful spintronic material, especially for its semiconductor compatibility.",2111.05417v1 2022-01-18,In-plane magnetic structure and exchange interactions in the high-temperature antiferromagnet Cr2Al,"The ordered tetragonal intermetallic Cr$_2$Al forms the same structure type as Mn$_2$Au, and the latter has been heavily investigated for its potential in antiferromagnetic spintronics due to its degenerate in-plane N\'{e}el vector. We present the single crystal flux growth of Cr$_2$Al and orientation-dependent magnetic properties. Powder neutron diffraction of Cr$_2$Al and first-principles simulations reveal that the magnetic ordering is likely in-plane and therefore identical to Mn$_2$Au, providing a second material candidate in the MoSi$_2$ structure type to evaluate the fundamental interactions that govern spintronic effects. The single ordering transition seen in thermal analysis and resistivity indicates that no canting of the moments along the $c$ axis is likely. Magnetometry, resistivity, and differential scanning calorimetry measurements confirm the N\'{e}el temperature to be $634 \pm 2$ K. First-principles simulations indicate that the system has a small density of states at the Fermi energy and confirm the lowest-energy magnetic ground state ordering, while Monte Carlo simulations match the experimental N\'{e}el temperature.",2201.07356v1 2024-03-26,Large topological Hall effect arising from spin reorientation in kagome magnet Fe3Ge,"Materials systems with spin chirality can provide ultra-high-density, ultra-fast, and ultralow-power information carriers for digital transformation. These material systems include magnetic skyrmions, chiral domain walls, spin reorientation,and so on. The topological Hall effect (THE) has been identified as the most convenient and effective tool for detecting the presence of spin chirality in these systems. The research on the THE that may arise from spin reorientation and specifically in Fe3Ge with spin reorientation remains an unexplored area, so we study the THE in Fe3Ge Conduct systematic research. X-Ray Diffraction (XRD) results indicate that our Fe3Ge ribbon sample has a D019 structure. First-principles calculations and magnetic and electrical testing confirm spin reorientation in the Fe3Ge ribbon sample at 350 K.The Hall resistivity test results are consistent with our expectations, indicating the presence of the THE in the Fe3Ge ribbon sample. The topological Hall resistivity reaches a maximum value of 0.69 m{\Omega} cm at 400 K. For the first time, a detailed experimental study of the THE in Fe3Ge with spin reorientation has been conducted, introducing a new member to the family of THE.",2403.17354v1 2022-08-23,Anomalous electrical transport and magnetic skyrmions in Mn-tuned Co9Zn9Mn2 single crystals,"\b{eta}-Mn-type CoxZnyMnz (x + y + z = 20) alloys have recently attracted increasing attention as a new class of chiral magnets with skyrmions at and above room temperature. However, experimental studies on the transport properties of this material are scarce. In this work, we report the successful growth of the \b{eta}-Mn-type Co9.24Zn9.25Mn1.51 and Co9.02Zn9.18Mn1.80 single crystals and a systematic study on their magnetic and transport properties. The skyrmion phase was found in a small temperature range just below the Curie temperature. The isothermal ac susceptibility and dc magnetization as a function of magnetic field confirm the existence of the skyrmion phase. A negative linear magnetoresistance over a wide temperature range from 2 K to 380 K is observed and attributed to the suppression of the magnetic ordering fluctuation under high fields. Both the magnetization and electrical resistivity are almost isotropic. The quantitative analysis of the Hall resistance suggests that the anomalous Hall effect of Co9.24Zn9.25Mn1.51 and Co9.02Zn9.18Mn1.80 single crystals is dominated by the intrinsic mechanism. Our findings contribute to a deeper understanding of the properties of CoxZnyMnz (x + y + z = 20) alloys material and advance their application in spintronic devices.",2208.10955v1 2007-08-31,Fundamental Constants,"The notion of ``fundamental constant'' is heavily theory-laden. A natural, fairly precise formulation is possible in the context of the standard model (here defined to include gravity). Some fundamental constants have profound geometric meaning. The ordinary gravitational constant parameterizes the stiffness, or resistance to curvature, of space-time. The cosmological term parameterizes space-time's resistance to expansion -- which may be, and apparently is at present, a {\it negative} resistance, i.e. a tendency toward expansion. The three gauge couplings of the strong, electromagnetic, and weak interactions parameterize resistance to curvature in internal spaces. The remaining fundamental couplings, of which there are a few dozen, supply an ungainly accommodation of inertia. The multiplicity and variety of fundamental constants are esthetic and conceptual shortcomings in our present understanding of foundational physics. I discuss some ideas for improving the situation. I then briefly discuss additional constants, primarily cosmological, that enter into our best established present-day world model. Those constants presently appear as macroscopic state parameters, i.e. as empirical ``material constants'' of the Universe. I mention a few ideas for how they might become fundamental constants in a future theory. In the course of this essay I've advertised several of my favorite speculations, including a few that might be tested soon.",0708.4361v1 2014-02-10,Tuning the band gap of PbCrO4 through high-pressure: Evidence of wide-to-narrow semiconductor transitions,"The electronic transport properties and optical properties of lead(II) chromate (PbCrO4) have been studied at high pressure by means of resistivity, Hall-effect, and optical-absorption measurements. Band-structure first-principle calculations have been also performed. We found that the low-pressure phase is a direct band-gap semiconductor (Eg = 2.3 eV) that shows a high resistivity. At 3.5 GPa, associated to a structural phase transition, a band-gap collapse takes place, becoming Eg = 1.8 eV. At the same pressure the resistivity suddenly decreases due to an increase of the carrier concentration. In the HP phase, PbCrO4 behaves as an n-type semiconductor, with a donor level probably associated to the formation of oxygen vacancies. At 15 GPa a second phase transition occurs to a phase with Eg = 1.2 eV. In this phase, the resistivity increases as pressure does probably due to the self-compensation of donor levels and the augmentation of the scattering of electrons with ionized impurities. In the three phases the band gap red shifts under compression. At 20 GPa, Eg reaches a value of 0.8 eV, behaving PbCrO4 as a narrow-gap semiconductor.",1402.2139v1 2015-08-11,Pressure induced electronic topological transition in Sb2S3,"Pressure induced electronic topological transitions in the wide band gap semiconductor Sb2S3 (Eg = 1.7-1.8 eV) with similar crystal symmetry (SG: Pnma) to its illustrious analog, Sb2Se3, has been studied using Raman spectroscopy, resistivity and the available literature on the x-ray diffraction studies. In this report, the vibrational and the transport properties of Sb2S3 have been studied up to 22 GPa and 11 GPa, respectively. We observed the softening of phonon modes Ag(2), Ag(3) and B2g and a sharp anomaly in their line widths at 4 GPa. The resistivity studies also shows an anomaly around this pressure. The changes in resistivity as well as Raman line widths can be ascribed to the changes in the topology of the Fermi surface which induces the electron-phonon and the strong phonon-phonon coupling, indicating a clear evidence of the electronic topological transition (ETT) in Sb2S3. The pressure dependence of a/c ratio plot obtained from the literature showed a minimum at ~ 5 GPa, which is consistent with our high pressure Raman and resistivity results. Finally, we give the plausible reasons for the non-existence of a non-trivial topological state in Sb2S3 at high pressures.",1508.02516v1 2018-11-19,Room-temperature Low-field Colossal Magneto-resistance in Double-perovskite Manganite,"The gigantic decrease of resistance by an applied magnetic field, which is often referred to as colossal magnetoresistance (CMR), has been an attracting phenomenon in strongly correlated electron systems. The discovery of CMR in manganese oxide compounds has developed the science of strong coupling among charge, orbital, and spin degrees of freedom. CMR is also attracting scientists from the viewpoint of possible applications to sensors, memories, and so on. However, no application using CMR effect has been achieved so far, partly because the CMR materials which satisfy all of the required conditions for the application, namely, high operating temperature, low operating magnetic field, and sharp resistive change, have not been discovered. Here we report a resistance change of more than two-orders of magnitude at a magnetic field lower than 2 T near 300 K in an A-site ordered NdBaMn_2_O_6_ crystal. When temperature and a magnetic field sweep from insulating (metallic) phase to metallic (insulating) phase, the insulating (metallic) conduction changes to the metallic (insulating) conduction within 1 K and 0.5 T, respectively. The CMR is ascribed to the melting of the charge ordering. The entropy change which is estimated from the B-T phase diagram is smaller than what is expected for the charge and orbital ordering. The suppression of the entropy change is attributable to the loss of the short range ferromagnetic fluctuation of Mn spin moments, which an important key of the high temperature and low magnetic field CMR effect.",1811.07596v1 2018-10-17,Perspectives of HgTe Topological Insulators for Quantum Hall Metrology,"We report the studies of high-quality HgTe/(Cd,Hg)Te quantum wells (QWs) with a width close to the critical one $d_c$, corresponding to the topological phase transition and graphene like band structure in view of their applications for Quantum Hall Effect (QHE) resistance standards. We show that in the case of inverted band ordering, the coexistence of conducting topological helical edge states together with QHE chiral states degrades the precision of the resistance quantization. By experimental and theoretical studies we demonstrate how one may reach very favorable conditions for the QHE resistance standards: low magnetic fields allowing to use permanent magnets ( B $\leq$ 1.4T) and simultaneously realtively high teperatures (liquid helium, T $\geq$ 1.3K). This way we show that HgTe QW based QHE resistance standards may replace their graphene and GaAs counterparts and pave the way towards large scale fabrication and applications of QHE metrology devices.",1810.07449v1 2019-07-25,Reducing sheet resistance of self-assembled transparent graphene films by defect patching and doping with UV/ozone treatment,"Liquid phase exfoliation followed by Langmuir-Blodgett self-assembly (LBSA) is a promising method for scalable production of thin graphene films for transparent conductor applications. However, monolayer assembly into thin films often induces a high density of defects, resulting in a large sheet resistance that hinders practical use. We introduce UV/ozone as a novel photochemical treatment that reduces sheet resistance of LBSA graphene threefold, while preserving the high optical transparency. The effect of such treatment on our films is opposite to the effect it has on mechanically exfoliated or CVD films, where UV/ozone creates additional defects in the graphene plane, increasing sheet resistance. Raman scattering shows that exposure to UV/ozone reduces the defect density in LBSA graphene, where edges are the dominant defect type. FTIR spectroscopy indicates binding of oxygen to the graphene lattice during exposure to ozone. In addition, work function measurements reveal that the treatment dopes the LBSA film, making it more conductive. Such defect patching paired with doping leads to an accessible way of improving the transparent conductor performance of LBSA graphene, making solution-processed thin films a candidate for industrial use.",1907.10916v2 2019-10-17,Link between magnetism and resistivity upturn in cuprates: a thermal conductivity study of La$_{2-x}$Sr$_x$CuO$_4$,"A key unexplained feature of cuprate superconductors is the upturn in their normal state electrical resistivity $\rho(T)$ seen at low temperature inside the pseudogap phase. We examined this issue via measurements of the thermal conductivity $\kappa(T)$ down to 50 mK and in fields up to 17 T on the cuprate La$_{2-x}$Sr$_x$CuO$_4$ at dopings $p = 0.13$, 0.136, 0.143 and 0.18. At $p$ = 0.136, 0.143, and 0.18, we observe an initial increase of the electronic thermal conductivity $\kappa_0/T$ as a function of field, as expected in a $d$-wave superconductor. For $p$ = 0.136 and 0.143, further increasing the field then leads to a decrease of $\kappa_0/T$, which correlates with the onset of spin density-wave order as observed in neutron scattering experiments on the same samples. This decrease of $\kappa_0/T$ with field is imposed by the Wiedemann-Franz law and the high value of the resistivity in the high-field normal state of these samples. Our study therefore provides a direct link between magnetism and the resistivity upturn in the pseudogap phase of cuprates. We discuss this scenario in the broader context of other cuprates.",1910.08126v1 2021-08-18,High Entropy Alloy CrFeNiCoCu sputtered films,"High entropy alloy(HEA) films of CrFeCoNiCu were prepared by sputtering, their structure was characterized, and their electric properties measured by temperature dependent Hall and Seebeck measurement. The HEA films show a solid solution with fcc structure, and a 111 texture with columnar grains of widths 15-30 nm extending through film thickness with very many twins. The residual electrical resistivity of the films is around 140 {\mu}{\Omega}cm and the temperature dependence of the resistivity is metal-like. The temperature coefficient of resistivity (TCR) is small (2 ppm/K). The Hall coefficient is positive while the Seebeck coefficients is negative. This is interpreted as arising from an electronic structure where the Fermi level passes through band states having both holes and electrons as indicated by band structure calculations. The HEA structure appears stable for annealing in vacuum, while annealing in an oxygen containing atmosphere causes the surface to oxidize and grow a Cr-rich oxide on the surface. This is then accompanied by demixing of the HEA solid solution and a decrease in residual resistance of the film.",2108.08373v2 2022-05-03,Structural and electronic phase transitions in Zr$_{1.03}$Se$_{2}$ at high pressure,"A detailed high pressure investigation is carried out using x-ray diffraction, Raman spectroscopy and low temperature resistivity measurements on hexagonal ZrSe$_{2}$ having an excess of 3 at.\% Zr. Structural studies show that the sample goes through a gradual structural transition from hexagonal to monoclinic phase, with a mixed phase in the pressure range 5.9 GPa to 14.8 GPa. Presence of a minimum in the $c/a$ ratio in the hexagonal phase and a minimum in the full width half maximum of the $A_{1g}$ mode at about the same pressure indicates an electronic phase transition. The sample shows a metallic characteristic in its low temperature resistivity data at ambient pressure, which persist till about 5.1 GPa and can be related the presence of slight excess Zr. At and above 7.3 GPa, the sample shows a metal to semiconductor transition with the opening of a very small band gap, which increases with pressure. The low temperature resistivity data show an upturn, which flattens with an increase in pressure. The phenomenological analysis of the low temperature resistivity data indicates the presence of Kondo effect in the sample, which may be due to the excess Zr.",2205.01322v1 2022-06-08,Quantized anomalous Hall resistivity achieved in molecular beam epitaxy-grown MnBi2Te4 thin films,"The intrinsic magnetic topological insulator MnBi2Te4 provides a feasible pathway to high temperature quantum anomalous Hall (QAH) effect as well as various novel topological quantum phases. Although quantized transport properties have been observed in exfoliated MnBi2Te4 thin flakes, it remains a big challenge to achieve molecular beam epitaxy (MBE)-grown MnBi2Te4 thin films even close to the quantized regime. In this work, we report the realization of quantized anomalous Hall resistivity in MBE-grown MnBi2Te4 thin films with the chemical potential tuned by both controlled in-situ oxygen exposure and top gating. We find that elongated post-annealing obviously elevates the temperature to achieve quantization of the Hall resistivity, but also increases the residual longitudinal resistivity, indicating a picture of high-quality QAH puddles weakly coupled by tunnel barriers. These results help to clarify the puzzles in previous experimental studies on MnBi2Te4 and to find a way out of the big difficulty in obtaining MnBi2Te4 samples showing quantized transport properties.",2206.03773v2 2022-07-23,Anomalous resistivity upturn in the van der Waals ferromagnet Fe$_5$GeTe$_2$,"Fe$_5$GeTe$_2$ (n = 3, 4, 5) have recently attracted increasing attention due to their two-dimensional van der Waals characteristic and high temperature ferromagnetism, which make promises for spintronic devices. The Fe(1) split site is one important structural characteristic of Fe$_5$GeTe$_2$ which makes it very different from other Fe$_5$GeTe$_2$ (n = 3, 4) systems. The local atomic disorder and short-range order can be induced by the split site. In this work, the high-quality van der Waals ferromagnet Fe$_5$GeTe$_2$ were grown to study the low-temperature transport properties. We found a resistivity upturn below 10 K. The temperature and magnetic field dependence of the resistivity are in good agreement with a combination of the theory of disorder-enhanced three-dimensional electron-electron and single-channel Kondo effect. The Kondo effect exists only at low magnetic field B < 3 T, while electron-electron dominates the appearance for the low-temperature resistivity upturn. We believe that the enhanced three-dimensional electron-electron interaction in this system is induced by the local atomic structural disorder due to the split site of Fe(1). Our results indicate that the split site of Fe plays an important role for the exceptional transport properties.",2207.11383v1 2000-09-21,High-pressure study of the non-Fermi liquid material U_2Pt_2In,"The effect of hydrostatic pressure (p<= 1.8 GPa) on the non-Fermi liquid state of U_2Pt_2In is investigated by electrical resistivity measurements in the temperature interval 0.3-300 K. The experiments were carried out on single-crystals with the current along (I||c) and perpendicular (I||a) to the tetragonal axis. The pressure effect is strongly current-direction dependent. For I||a we observe a rapid recovery of the Fermi-liquid T^2-term with pressure. The low-temperature resistivity can be analysed satisfactorily within the magnetotransport theory of Rosch, which provides strong evidence for the location of U_2Pt_2In at an antiferromagnetic quantum critical point. For I||c the resistivity increases under pressure, indicating the enhancement of an additional scattering mechanism. In addition, we have measured the pressure dependence of the antiferromagnetic ordering temperature (T_N= 37.6 K) of the related compound U_2Pd_2In. A simple Doniach-type diagram for U_2Pt_2In and U_2Pd_2In under pressure is presented.",0009324v1 2002-04-19,Spin-injection through an Fe/InAs Interface,"The spin-dependence of the interface resistance between ferromagnetic Fe and InAs is calculated from first-principles for specular and disordered (001) interfaces. Because of the symmetry mismatch in the minority-spin channel, the specular interface acts as an efficient spin filter with a transmitted current polarisation between 98 an 89%. The resistance of a specular interface in the diffusive regime is comparable to the resistance of a few microns of bulk InAs. Symmetry-breaking arising from interface disorder reduces the spin asymmetry substantially and we conclude that efficient spin injection from Fe into InAs can only be realized using high quality epitaxial interfaces.",0204422v1 2002-10-01,Free and Trapped Injected Carriers in C60 Crystals,"We report on the conductance from two-contact carrier injection in C60 single crystals. In the nonlinear regime, the current and voltage obey a power law, I \~ V^m, where m can be as high as 10 at room temperature. This nonlinear behavior - the resistance decreases by 6 orders of magnitude without saturation - is among the highest reported for organic systems, and can be explained by injection of free carriers into the trap-filling region. We find that H2 annealing suppresses shallow traps and enhances nonlinearity. Two limiting types of temperature dependence of the nonlinear resistance are observed - decreasing and increasing resistance at the orientational ordering temperature. A simple model incorporating deep traps is presented to understand this behavior and the impact of this model on possible field-effect transistor action is discussed.",0210029v1 2003-02-03,Critical Current Density and Resistivity of MgB2 Films,"The high resistivity of many bulk and film samples of MgB2 is most readily explained by the suggestion that only a fraction of the cross-sectional area of the samples is effectively carrying current. Hence the supercurrent (Jc) in such samples will be limited by the same area factor, arising for example from porosity or from insulating oxides present at the grain boundaries. We suggest that a correlation should exist, Jc ~ 1/{Rho(300K) - Rho(50K)}, where Rho(300K) - Rho(50K) is the change in the apparent resistivity from 300 K to 50 K. We report measurements of Rho(T) and Jc for a number of films made by hybrid physical-chemical vapor deposition which demonstrate this correlation, although the ""reduced effective area"" argument alone is not sufficient. We suggest that this argument can also apply to many polycrystalline bulk and wire samples of MgB2.",0302017v1 2003-03-19,Structural and Electronic Properties of Amorphous and Polycrystalline In2Se3 Films,"Structural and electronic properties of amorphous and single-phase polycrystalline films of gamma- and kappa-In2Se3 have been measured. The stable gamma phase nucleates homogeneously in the film bulk and has a high resistivity, while the metastable kappa phase nucleates at the film surface and has a moderate resistivity. The microstructures of hot-deposited and post-annealed cold-deposited gamma films are quite different but the electronic properties are similar. The increase in the resistivity of amorphous In2Se3 films upon annealing is interpreted in terms of the replacement of In-In bonds with In-Se bonds during crystallization. Great care must be taken in the preparation of In2Se3 films for electrical measurements as the presence of excess chalcogen or surface oxidation may greatly affect the film properties.",0303369v1 2003-04-16,Initial dissipation and current-voltage characteristics of superconductors containing fractal clusters of a normal phase,"The influence of fractal clusters of a normal phase on distinctive features of current-voltage characteristic of percolative type-II superconductors is considered. The results of high-resolution measurements of the differential resistance of BPSCCO/Ag composites are discussed in the context of magnetic flux dynamics. The region of initial dissipation is observed on current-voltage characteristics in the neighborhood of the transition into a resistive state. In the course of this stage of resistive transition the vortices start to break away from the normal-phase clusters, which act as pinning centers. The effect of transport current on vortex depinning is investigated. A broad current range of initial dissipation is considered as an evidence of fractal nature of the normal-phase clusters.",0304354v2 2003-12-12,Electronic behavior in mats of single-walled carbon nanotubes under pressure,"Single-walled carbon nanotubes (SWNTs) have many interesting properties; they may be metallic or semiconducting depending on their diameter and helicity of the graphene sheet. Hydrostatic or quasi-hydrostatic high pressures can probe many electronic features. Resistance - temperature measurements in SWNTs from normal condition and under 0.4 GPa of quasi-hydrostatic pressures reveal a semiconducting-like behavior. From 0.5 to about 2.0 GPa the resistance changes to a Kondo-like feature due to magnetic impurities used to catalyse the nanotube formation. Above 2.0 GPa, they become metallic and at about 2.4 GPa the resistance decreases dramatically around 3 K suggesting a superconducting transition.",0312307v1 2004-08-12,Impedance spectroscopy study on post-annealing-tuned polycrystalline CaCu3Ti4O12 films: Evidence of Barrier Layer Capacitor Effects,"In this paper, impedance spectroscopy study was performed to establish the electrical property and microstructure relations of the as-deposited and post-annealed polycrystalline CCTO films prepared on Pt/Ti/SiO2/Si (100) substrates by pulsed-laser deposition (PLD). Our results demonstrated that the as-deposited polycrystalline CCTO film was made of insulating grain boundaries with semiconducting grains, indicating that the high-dielectric-constant is attributed to the barrier layer capacitor (BLC) effects. The simple resistor-capacitor (RC) equivalent circuit and the modified constant phase element (CPE) circuit were used to describe the impedance spectroscopy, and excellent agreement between the calculated and measured curves was obtained in the CPE circuit. The resistance and capacitance of the grains and grain boundaries can be tuned by changing the annealing atmosphere and temperature. Under oxygen-absent annealing atmosphere, the electric resistances of the grain boundaries changed greatly but the resistance of the grains has almost no change. While under oxygen annealing atmosphere, the reverse happened. On the basis of this result, it is demonstrated that the origin of the semiconductivity of the grains in CCTO polycrystalline films arises from their oxygen-loss, while the grain boundaries are close to oxygen- stoicheometry.",0408275v2 2004-12-03,Resistance noise scaling in a 2D system in GaAs,"The 1/f resistance noise of a two-dimensional (2D) hole system in a high mobility GaAs quantum well has been measured on both sides of the 2D metal-insulator transition (MIT) at zero magnetic field (B=0), and deep in the insulating regime. The two measurement methods used are described: I or V fixed, and measurement of resp. V or I fluctuations. The normalized noise magnitude SR/R^2 increases strongly when the hole density is decreased, and its temperature (T) dependence goes from a slight increase with T at the largest densities, to a strong decrease at low density. We find that the noise magnitude scales with the resistance, SR /R^2 ~ R^2.4. Such a scaling is expected for a second order phase transition or a percolation transition. The possible presence of such a transition is investigated by studying the dependence of the conductivity as a function of the density. This dependence is consistent with a critical behavior close to a critical density p* lower than the usual MIT critical density pc.",0412084v1 2005-10-21,"Superconductivity mediated by a soft phonon mode: specific heat, resistivity, thermal expansion and magnetization of YB6","The superconductor YB6 has the second highest critical temperature Tc among the boride family MBn. We report measurements of the specific heat, resistivity, magnetic susceptibility and thermal expansion from 2 to 300 K, using a single crystal with Tc = 7.2 K. The superconducting gap is characteristic of medium-strong coupling. The specific heat, resistivity and expansivity curves are deconvolved to yield approximations of the phonon density of states, the spectral electron-phonon scattering function and the phonon density of states weighted by the frequency-dependent Grueneisen parameter respectively. Lattice vibrations extend to high frequencies >100 meV, but a dominant Einstein-like mode at ~8 meV, associated with the vibrations of yttrium ions in oversized boron cages, appears to provide most of the superconducting coupling and gives rise to an unusual temperature behavior of several observable quantities. A surface critical field Hc3 is also observed.",0510572v3 2006-03-31,Evidences of a consolute critical point in the Phase Separation regime of La(5/8-y)Pr(y)Ca(3/8)MnO(3) (y = 0.4) single crystals,"We report on DC and pulsed electric field sensitivity of the resistance of mixed valent Mn oxide based La(5/8-y)Pr(y)Ca(3/8)MnO(3) (y = 0.4) single crystals as a function of temperature. The low temperature regime of the resistivity is highly current and voltage dependent. An irreversible transition from high (HR) to a low resistivity (LR) is obtained upon the increase of the electric field up to a temperature dependent critical value (V_c). The current-voltage characteristics in the LR regime as well as the lack of a variation in the magnetization response when V_c is reached indicate the formation of a non-single connected filamentary conducting path. The temperature dependence of V_c indicates the existence of a consolute point where the conducting and insulating phases produce a critical behavior as a consequence of their separation.",0603850v1 2007-06-29,NMR relaxation and resistivity from rattling phonons in pyrochlore superconductors,"We calculate the temperature dependence of NMR relaxation rate and electrical resistivity for coupling to a local, strongly anharmonic phonon mode. We argue that the two-phonon Raman process is dominating NMR relaxation. Due to the strong anharmonicity of the phonon an unusual temperature dependence is found having a low temperature peak and becoming constant towards higher temperatures. The electrical resistivity is found to vary like T^2 at low temperatures and following a sqrt{T} behavior at high temperatures. Both results are in qualitative agreement with recent observations on beta-pyrochlore oxide superconductors.",0706.4345v2 2007-07-04,NaV2O4: a Quasi-1D Metallic Antiferromagnet with Half-Metallic Chains,"NaV2O4 crystals were grown under high pressure using a NaCl flux, and the crystals were characterized with X-ray diffraction, electrical resistivity, heat capacity, and magnetization. The structure of NaV2O4 consists of double chains of edge-sharing VO6 octahedra. The resistivity is highly anisotropic, with the resistivity perpendicular to the chains more than 20 times greater than that parallel to the chains. Magnetically, the intrachain interactions are ferromagnetic and the interchain interactions are antiferromagnetic; 3D antiferromagnetic order is established at 140 K. First principles electronic structure calculations indicate that the chains are half metallic. Interestingly, the case of NaV2O4 seems to be a quasi-1D analogue of what was found for half-metallic materials.",0707.0519v3 2007-09-11,Transport properties and magnetic field induced localization in the misfit cobaltite [Bi$_2$Ba$_{1.3}$K$_{0.6}$Co$_{0.1}$]$^{RS}$[CoO$_2$]$_{1.97}$ single crystal,"Resistivity under magnetic field, thermopower and Hall coefficient are systematically studied for [Bi$_2$Ba$_{1.3}$K$_{0.6}$Co$_{0.1}$]$^{RS}$[CoO$_2$]$_{1.97}$ single crystal. In-plane resistivity ($\rho_{ab}$(T)) shows metallic behavior down to 2 K with a $T^2$ dependence below 30 K; while out-of-plane resistivity ($\rho_{c}(T)$) shows metallic behavior at high temperature and a thermal activation semiconducting behavior below about 12 K. Striking feature is that magnetic field induces a ln(1/$T$) diverging behavior in both $\rho_{ab}$ and $\rho_{c}(T)$ at low temperature. The positive magnetoresistance (MR) could be well fitted by the formula based on multi-band electronic structure. The ln(1/$T$) diverging behavior in $\rho_{ab}$ and $\rho_{c}(T)$ could arise from the magnetic-field-induced 2D weak localization or spin density wave.",0709.1519v1 2007-11-29,Magnetoelectric Effects on Composite Nano Granular $Fe/TiO_{2-δ}$ Films,"Employing a new experimental technique to measure magnetoelectric response functions, we have measured the magnetoelectric effect in composite films of nano granular metallic iron in anatase titanium dioxide at temperatures below 50 K. A magnetoelectric resistance is defined as the ratio of a transverse voltage to bias current as a function of the magnetic field. In contrast to the anomalous Hall resistance measured above 50 K, the magnetoelectic resistance below 50 K is significantly larger and exhibits an even symmetry with respect to magnetic field reversal $H\to -H$. The measurement technique required attached electrodes in the plane of the film composite in order to measure voltage as a function of bias current and external magnetic field. To our knowledge, the composite films are unique in terms of showing magnetoelectric effects at low temperatures, $<$ 50 K, and anomalous Hall effects at high temperatures, $>$ 50 K.",0711.4776v1 2009-04-23,Microscopic origin of bipolar resistive switching of nanoscale titanium oxide thin films,"We report a direct observation of the microscopic origin of the bipolar resistive switching behavior in nanoscale titanium oxide films. Through a high-resolution transmission electron microscopy, an analytical TEM technique using energy-filtering transmission electron microscopy and an in situ x-ray photoelectron spectroscopy, we demonstrated that the oxygen ions piled up at top interface by an oxidation-reduction reaction between the titanium oxide layer and the top Al metal electrode. We also found that the drift of oxygen ions during the on/off switching induced the bipolar resistive switching in the titanium oxide thin films.",0904.3628v2 2009-08-25,"Bipolar resistive switching characteristics of poly(3,4-ethylene-dioxythiophene): poly(styrenesulfonate) thin film","We investigated the reversible resistive switching of poly(3,4-ethylenedioxythiophene):polystyrenesulfonate (PEDOT:PSS) thin films sandwiched between Al electrodes. The J-V sweep curve showed a hysteretic behavior which depends on the polarity of the applied voltage bias. From the analysis of I-V curves, it was revealed that the charge transport through the junction was governed by the bulk space-charge-limited conduction (SCLC) model. Using transmission electron microscopy (TEM) analysis, it was confirmed that the initial high resistance state of PEDOT:PSS films is related with the segregation of PSS- chains induced by redox reaction between a Al metal electrode and PEDOT:PSS film. Positive space charges present on the top region of PEDOT:PSS films can be proposed as a possible trap centers of electron trapping and detrapping process.",0908.3527v1 2010-02-02,Memristor Behaviour in Nano-Sized Vertical Lsmo/Lsmo Tunnel Junctions,"We report a memory resistance (memristor) behavior with nonlinear current-voltage characteristics and bipolar hysteretic resistance switching in the nanocolumnar manganite (LSMO) films. The switching from a high (HRS) to a low (LRS) resistance occurs at a bias field ~1 MV/cm. Applied electric field drops mostly at the insulating interfacial LSMO layer and couples to correlated polarons at the LSMO(111)/LSMO(111) vertical interfaces. The observed memristance behaviour has an electronic (polaronic) origin and is caused by an electric-field-controlled Jahn-Teller (JT) effect, followed by the orbital reconstruction and formation of a metastable orbitally disordered interfacial phase (LRS). Compared to the earlier reported ionic memristor in Ti-O films, an electronic (polaronic) nano-sized LSMO memristor shows an additional (re-entrant) LRS-HRS switching at higher fields because of the second minimum in the elastic energy of a JT system.",1002.0495v1 2010-02-11,"Synthesis, anisotropy, and superconducting properties of LiFeAs single crystal","A LiFeAs single crystal with $T_c^{onset}$$\sim$19.7 K was grown successfully in a sealed tungsten crucible using the Bridgeman method. The electrical resistivity experiments revealed a ratio of room temperature to residual resistivity (RRR) of approximately 46 and 18 for the in-plane and out-of plane directions. The estimated anisotropic resistivity, $\gamma_\rho$=$\rho_c$ / $\rho_{ab}$, was approximately 3.3 at $T_c^{onset}$. The upper critical fields had large $H_{c2} ^{\shortparallel ab}$ and $H_{c2}^{\shortparallel c}$ values of 83.4 T and 72.5 T, respectively, and an anisotropy ratio is $\gamma_H$=$H_{c2}^{\shortparallel ab}$ / $H_{c2} ^{\shortparallel c}$$\sim$1.15. The high upper critical field value and small anisotropy highlight the potential use of LiFeAs in a variety of applications. The calculated critical current density $(J_c)$ from the $M$-$H$ loop is approximately 10$^3$ A/cm$^2$",1002.2249v1 2010-07-15,Role of interface reaction on resistive switching of Metal/a-TiO2/Al RRAM devices,"For the clear understanding of the role of interface reaction between top metal electrode and titanium oxide layer, we investigated the effects of various top metals on the resistive switching in Metal/a-TiO2/Al devices. The top Al device with the highest oxygen affinity showed the best memory performance, which is attributed to the fast formation of interfacial layer (Al-Ti-O), as confirmed by high resolution transmission electron microscopy and electron dispersive spectroscopy. Hence, we concluded that the interface layer, created by the redox reaction between top metal electrode and TiO2 layer, plays a crucial role in bipolar resistive switching behaviors of metal/TiO2/Al systems.",1007.2463v1 2010-11-05,Interplay between the electrical transport properties of GeMn thin films and Ge substrates,"We present evidence that electrical transport studies of epitaxial p-type GeMn thin films fabricated on high resistivity Ge substrates are severely influenced by parallel conduction through the substrate, related to the large intrinsic conductivity of Ge due to its small bandgap. Anomalous Hall measurements and large magneto resistance effects are completely understood by taking a dominating substrate contribution as well as the measurement geometry into account. It is shown that substrate conduction persists also for well conducting, degenerate, p-type thin films, giving rise to an effective two-layer conduction scheme. Using n-type Ge substrates, parallel conduction through the substrate can be reduced for the p-type epi-layers, as a consequence of the emerging pn-interface junction. GeMn thin films fabricated on these substrates exhibit a negligible magneto resistance effect. Our study underlines the importance of a thorough characterization and understanding of possible substrate contributions for electrical transport studies of GeMn thin films.",1011.1450v1 2011-08-31,Local Tunneling Magnetoresistance probed by Low-Temperature Scanning Laser Microscopy,"Tunneling magnetoresistance (TMR) in a vertical manganite junction was investigated by low-temperature scanning laser microscopy (LTSLM) allowing to determine the local relative magnetization M orientation of the two electrodes as a function of magnitude and orientation of the external magnetic field H. Sweeping the field amplitude at fixed orientation revealed magnetic domain nucleation and propagation in the junction electrodes. For the high-resistance state an almost single-domain antiparallel magnetization configuration was achieved, while in the low-resistance state the junction remained in a multidomain state. Calculated resistance $R_\mathrm{calc}(H)$ based on the local M configuration obtained by LTSLM is in quantitative agreement with R(H) measured by magnetotransport.",1108.6159v1 2012-04-16,Experimental investigation of the magnetic field driven superconductor/ insulator transition in underdoped $La_{2-x}Sr_xCuO_4$ thin films,"The magnetic field driven superconductor/insulator transition is studied in a large variety of $La_{2-x}Sr_xCuO_4$ thin films of various Sr dopings. Temperature dependence of the resistivity down to 4.2 or 1.5 K under high pulsed magnetic field (up to 57 T) is analyzed. In particular, the existence of plateaus in the resistance versus temperature curves, in a limited range of temperature, for given values of the magnetic field is carefully investigated. It is shown to be associated to scaling behaviour of the resistance versus magnetic field curves, evocative of the presence of a quantum critical point. A three-dimensional (H,x,T) phase diagram is proposed, taking into account the intrinsic lamellar nature of the materials by the existence of a temperature crossover from quantum-two-dimensional to three-dimensional behavior.",1204.3493v1 2012-08-20,Universal linear in temperature resistivity from black hole superradiance,"Observations across many families of unconventional materials motivative the search for robust mechanisms producing linear in temperature d.c. resistivity. BKT quantum phase transitions are commonplace in holographic descriptions of finite density matter, separating critical and ordered phases. We show that at a holographic BKT critical point, if the unstable operator is coupled to the current via irrelevant operators, then a linear contribution to the resistivity is universally obtained. We also obtain broad power law tails in the optical conductivity, that shift spectral weight from the Drude peak as well as interband energy scales. We give a partial realization of this scenario using an Einstein-Maxwell-pseudoscalar bulk theory. The instability is a vectorial mode at nonzero wavevector, which is communicated to the homogeneous current via irrelevant coupling to an ionic lattice.",1208.4102v1 2012-11-12,Magnetic and transport properties of tetragonal- or cubic-Heusler-type Co-substituted Mn-Ga epitaxial thin films,"The composition dependence of the structural, magnetic, and transport properties of epitaxially grown Mn-Co-Ga films were investigated. The crystal structure was observed to change from tetragonal to cubic as the Co content was increased. In terms of the dependence of saturation magnetization on the Co content, relatively small value was obtained for the Mn$_{2.3}$Co$_{0.4}$Ga$_{1.3}$ film at a large {\it K}$_\textrm u$ value of 9.2 Merg/cm$^3$. Electrical resistivity of Mn-Co-Ga films was larger than that of pure Mn-Ga film. The maximum value of the resistivity was 490 $\mu\Omega$cm for Mn$_{2.2}$Co$_{0.6}$Ga$_{1.2}$ film. The high resistivity of Mn-Co-Ga might be due to the presence of localized electron states in the films due to chemical disordering caused by the Co substitution.",1211.2524v1 2013-03-19,Self-Formation of Sub-10-nm Nanogaps by Silicidation for Resistive Switch in Air,"We developed a simple and reliable method for the fabrication of sub-10-nm wide nanogaps. The self-formed nanogap is based on the stoichiometric solid-state reaction between metal and Si atoms during silicidation process. The nanogap width is deter- mined by the metal layer thickness. Our proposed method produces nanogaps either symmetric or asymmetric electrodes, as well as, multiple nanogaps within one unique process step for application to complex circuits. Therefore, this method provides high throughput and it is suitable for large-scale production. To demonstrate the feasibil- ity of the proposed fabrication method, nanogap resistive switches have been built and characterized. They exhibit a pronounced hysteresis with up to 103 on/off conductance ratios in air. Our results indicate that the voltages for initially electroforming the de- vice to the switch state are determinated by the nanogap sizes. However, the set and reset voltages of the device do not strongly dependent on the nanogap widths. These phenomena could be helpful to understand how the resistive switching is established.",1303.4586v1 2013-10-13,Origin of the energy gap in the narrow-gap semiconductor FeSb2 revealed by high-pressure magnetotransport measurements,"To elucidate an origin of the two energy gaps in the narrow-gap semiconductor FeSb2, we have investigated the effects of hydrostatic pressure on the resistivity, Hall resistance and magnetoresistance at low temperatures. The larger energy gap evaluated from the temperature dependence of resistivity above 100 K is enhanced from 30 to 40 meV with pressure from 0 to 1.8 GPa, as generally observed in conventional semiconductors. In the low-temperature range where a large Seebeck coefficient was observed, we evaluate the smaller energy gap from the magnetotransport tensor using a two-carrier model and find that the smaller gap exhibits a weak pressure dependence in contrast to that of the larger gap. To explain the pressure variations of the energy gaps, we propose a simple model that the smaller gap is a gap from the impurity level to the conduction band and the larger one is a gap between the valence and conduction bands, suggesting that the observed large Seebeck coefficient is not relevant to electron correlation effects.",1310.3451v1 2013-10-30,Analysis of post wet chemistry heat treatment effects on Nb SRF surface resistance,"Most of the current research in superconducting radio frequency (SRF) cavities is focused on ways to reduce the construction and operating cost of SRF based accelerators as well as on the development of new or improved cavity processing techniques. The increase in quality factors is the result of the reduction of the surface resistance of the materials. A recent test on a 1.5 GHz single cell cavity made from ingot niobium of medium purity and heat treated at 1400 C in a ultra-high vacuum induction furnace resulted in a residual resistance of about 1nanoohm and a quality factor at 2.0 K increasing with field up to 5x10^10 at a peak magnetic field of 90 mT. In this contribution, we present some results on the investigation of the origin of the extended Q0-increase, obtained by multiple HF rinses, oxypolishing and heat treatment of all Nb cavities.",1310.8159v1 2014-02-04,Multilevel recording in Bi-deficient Pt/BFO/SRO heterostructures based on ferroelectric resistive switching targeting high-density information storage in nonvolatile memories,"We demonstrate the feasibility of multilevel recording in Pt/Bi(1-d)FeO3/SrRuO3 capacitors using the ferroelectric resistive switching phenomenon exhibited by the Pt/Bi(1-d)FeO3 interface. A tunable population of up and down ferroelectric domains able to modulate the Schottky barrier height at the Pt/Bi(1-d)FeO3 interface can be achieved by means of either a collection of SET/RESET voltages or current compliances. This programming scheme gives rise to well defined resistance states, which form the basis for a multilevel storage nonvolatile memory.",1402.0739v1 2014-05-06,Effect of realistic metal electronic structure on the lower limit of contact resistivity of epitaxial metal-semiconductor contacts,"The effect of realistic metal electronic structure on the lower limit of resistivity in [100] oriented n-Si is investigated using full band Density Functional Theory and Semi-Empirical Tight Binding (TB) calculations. Using simulation unit cells guided by the interface chemistry of epitaxial CoSi2 on [100] oriented Si observed experimentally, it is shown that the 'ideal metal' assumption fails in some situations and consequently underestimates the lower limit of contact resistivity in n-Si by at least an order of magnitude at high doping concentrations. The mismatch in transverse momentum space in the metal and the semiconductor, the so-called 'valley filtering effect', is shown to be dependent on the interface chemistry simulated. The results emphasize the need for explicit inclusion of the metal atomic and electronic structure in the atomistic modeling of transport across metal-semiconductor contacts",1405.1317v1 2014-11-16,Laser doping for ohmic contacts in n-type Ge,"We achieved ohmic contacts down to 5 K on standard n-doped Ge samples by creating a strongly doped thin Ge layer between the metallic contacts and the Ge substrate. Thanks to the laser doping technique used, Gas Immersion Laser Doping, we could attain extremely large doping levels above the solubility limit, and thus reduce the metal/doped Ge contact resistance. We tested independently the influence of the doping concentration and doped layer thickness, and showed that the ohmic contact improves when increasing the doping level and is not affected when changing the doped thickness. Furthermore, we characterised the doped Ge/Ge contact, showing that at high doping its contact resistance is the dominant contribution to the total contact resistance.",1411.4325v1 2015-02-19,Anomalous impact of hydrostatic pressure on superconductivity of polycrystalline LaO0.5F0.5BiSe2,"We report bulk superconductivity at 2.5K in LaO0.5F0.5BiSe2 compound through the DC magnetic susceptibility and electrical resistivity measurements. The synthesized LaO0.5F0.5BiSe2 compound is crystallized in tetragonal structure with space group P4/nmm and Reitveld refined lattice parameters are a= 4.15(1)A and c=14.02(2)A. The lower critical field of Hc1= 40Oe, at temperature 2K is estimated through the low field magnetization measurements. The LaO0.5F0.5BiSe2 compound showed metallic normal state electrical resistivity with residual resistivity value of 1.35m{\Omega}-cm. The compound is type-II superconductor, and the estimated Hc2(0) value obtained by WHH formula is above 20kOe for 90percent Rn criteria. The superconducting transition temperature decreases with applied pressure till around 1.68GPa and with further higher pressures a high Tc phase emerges with possible onset Tc of above 5K for 2.5GPa.",1502.05502v3 2016-06-13,Performance studies of MRPC prototypes for CBM,"Multi-gap Resistive Plate Chambers (MRPCs) with multi-strip readout are considered to be the optimal detector candidate for the Time-of-Flight (ToF) wall in the Compressed Baryonic Matter (CBM) experiment. In the R&D phase MRPCs with different granularities, low-resistive materials and high voltage stack configurations were developed and tested. Here, we focus on two prototypes called HD-P2 and THU-strip, both with strips of 27 cm$^2$ length and low-resistive glass electrodes. The HD-P2 prototype has a single-stack configuration with 8 gaps while the THU-strip prototype is constructed in a double-stack configuration with 2 $\times$ 4 gaps. The performance results of these counters in terms of efficiency and time resolution carried out in a test beam time with heavy-ion beam at GSI in 2014 are presented in this proceeding.",1606.04917v1 2016-06-28,Observation of quantum Hall effect in a microstrained Bi$_2$Se$_3$ single crystal,"We report the observation of quantum Hall effect (QHE) in a Bi$_2$Se$_3$ single crystal having carrier concentration ($n$) $\sim1.13\times10^{19}$cm$^{-3}$, three dimensional Fermi surface and bulk transport characteristics. The plateaus in Hall resistivity coincide with minima of Shubnikov de Haas oscillations in resistivity. Our results demonstrate that the presence of perfect two dimensional transport is not an essential condition for QHE in Bi$_2$Se$_3$. The results of high resolution x-ray diffraction (HRXRD), energy-dispersive x-ray spectroscopy (EDX), and residual resistivity measurements show the presence of enhanced crystalline defects and microstrain. We propose that the formation of localized state at the edge of each Landau level due to resonance between the bulk and defect band of Bi$_2$Se$_3$ causes the quantum Hall effect.",1606.08576v1 2016-07-20,Nonlocal topological valley transport at large valley Hall angles,"Berry curvature hot spots in two-dimensional materials with broken inversion symmetry are responsible for the existence of transverse valley currents, which give rise to giant nonlocal dc voltages. Recent experiments in high-quality gapped graphene have highlighted a saturation of the nonlocal resistance as a function of the longitudinal charge resistivity $\rho_{{\rm c}, xx}$, when the system is driven deep into the insulating phase. The origin of this saturation is, to date, unclear. In this work we show that this behavior is fully compatible with bulk topological transport in the regime of large valley Hall angles (VHAs). We demonstrate that, for a fixed value of the valley diffusion length, the dependence of the nonlocal resistance on $\rho_{{\rm c}, xx}$ weakens for increasing VHAs, transitioning from the standard $\rho^3_{{\rm c}, xx}$ power-law to a result that is independent of $\rho_{{\rm c}, xx}$.",1607.05902v1 2016-10-26,Resistive Switching and Voltage Induced Modulation of Tunneling Magnetoresistance in Nanosized Perpendicular Organic Spin Valves,"Nanoscale multifunctional perpendicular organic spin valves have been fabricated. The devices based on an La$_{0.7}$Sr$_{0.3}$MnO$_3$/Alq$_3$/Co trilayer show resistive switching of up to 4-5 orders of magnitude and magnetoresistance as high as -70% the latter even changing sign when voltage pulses are applied. This combination of phenomena is typically observed in multiferroic tunnel junctions where it is attributed to magnetoelectric coupling between a ferromagnet and a ferroelectric material. Modeling indicates that here the switching originates from a modification of the La$_{0.7}$Sr$_{0.3}$MnO$_3$ surface. This modification influences the tunneling of charge carriers and thus both the electrical resistance and the tunneling magnetoresistance which occurs at pinholes in the organic layer.",1610.08218v1 2016-11-03,Current crowding mediated large contact noise in graphene field-effect transistors,"The impact of the intrinsic time-dependent fluctuations in the electrical resistance at the graphene-metal interface or the contact noise, on the performance of graphene field effect transistors, can be as adverse as the contact resistance itself, but remains largely unexplored. Here we have investigated the contact noise in graphene field effect transistors of varying device geometry and contact configuration, with carrier mobility ranging from 5,000 to 80,000$~$cm$^{2}$V$^{-1}$s$^{-1}$. Our phenomenological model for contact noise due to current crowding in purely two dimensional conductors, confirms that the contacts dominate the measured resistance noise in all graphene field effect transistors in the two-probe or invasive four probe configurations, and surprisingly, also in nearly noninvasive four probe (Hall bar) configuration in the high mobility devices. The microscopic origin of contact noise is directly linked to the fluctuating electrostatic environment of the metal-channel interface, which could be generic to two dimensional material-based electronic devices.",1611.01181v2 2017-09-02,Signatures of the Kondo effect in VSe2,"VSe2 is a transition metal dichaclogenide which has a charge-density wave transition that has been well studied. We report on a low-temperature upturn in the resistivity and, at temperatures below this resistivity minimum, an unusual magnetoresistance which is negative at low fields and positive at higher fields, in single crystals of VSe2. The negative magnetoresistance has a parabolic dependence on the magnetic field and shows little angular dependence. The magnetoresistance at temperatures above the resistivity minimum is always positive. We interpret these results as signatures of the Kondo effect in VSe2. An upturn in the susceptibility indicates the presence of interlayer V ions which can provide the localized magnetic moments required for scattering the conduction electrons in the Kondo effect. The low-temperature behaviour of the heat capacity, including a high value of gamma, along with a deviation from a Curie-Weiss law observed in the low-temperature magnetic susceptibility, are consistent with the presence of magnetic interactions between the paramagnetic interlayer V ions and a Kondo screening of these V moments.",1709.00594v1 2017-11-20,Computational analysis of short-range interactions between an edge dislocation and an array of equally-spaced identical shearable or non-shearable precipitates,"The interaction between dislocations and precipitates plays an important role in the mechanical behavior of alloys. To provide more insight into the physics of this interaction, this research analyzes short-range interactions of an edge dislocation with an array of equally-spaced identical precipitates. We use a modified dislocation dynamics approach accounting for penetrable and impenetrable precipitates. This research quantifies the effects of precipitate resistance on the geometry of the dislocation-precipitation interaction and the local distribution of plastic strain near a precipitate. The results show that a precipitate with a higher resistance causes an increase in the maximum value of dislocation curvature during the bypass. In addition, a higher level of precipitate resistance leads to a lower level of plastic deformation. Moreover, we observed a high plastic strain gradient at the interface of non-shearable precipitates.",1711.07428v2 2018-01-25,Non-volatile bipolar resistive switching in sol-gel derived BiFeO3 thin films,"BiFeO3 thin films are deposited on FTO coated glass substrates using a simple sol-gel deposition technique, limiting thickness about 70 nm and Ag/BiFeO3/FTO RRAM devices are prepared. The devices showed low-voltage bipolar switching with the maximum Ion/Ioff ~ 450, and low set and reset voltages ~ 1.1 V and -1.5 V, respectively. The devices are stable against on-off cycles with ~ 104 s retention time without any significant degradation. The variations in the set and reset voltages are 0.4 V and 0.6 V, respectively. We found that ohmic and trap-controlled space charge limited conductions are responsible for low and high resistance states, respectively. The resistive switching mechanism is attributed to the formation and rupturing of the metal filament during the oxidation and reduction of Ag ions for the set and reset states.",1801.08502v1 2017-03-22,A comparative study of resists and lithographic tools using the Lumped Parameter Model,"A comparison of the performance of high resolution lithographic tools is presented here. We use extreme ultraviolet interference lithography, electron beam lithography, and He ion beam lithography tools on two different resists that are processed under the same conditions. The dose-to-clear and the lithographic contrast are determined experimentally and are used to compare the relative efficiency of each tool. The results are compared to previous studies and interpreted in the light of each tool-specific secondary electron yield. In addition, the patterning performance is studied by exposing dense line/spaces patterns and the relation between critical dimension and exposure dose is discussed. Finally, the Lumped Parameter Model is employed in order to quantitatively estimate the critical dimension of line/spaces, using each tool specific aerial image. Our implementation is then validated by fitting the model to the experimental data from interference lithography exposures, and extracting the resist contrast.",1703.08229v1 2020-04-15,Radiation reaction friction: Resistive material medium,"We explore a novel method of describing the radiation friction of particles traveling through a mechanically resistive medium. We introduce a particle motion induced matter warping along the path in a manner assuring that charged particle dynamics occurs subject to radiative energy loss described by the Larmor formula. We compare our description with the Landau-Lifshitz-like model for the radiation friction and show that the established model exhibits non-physical behavior. Our approach predicts in the presence of large mechanical friction an upper limit on radiative energy loss being equal to the energy loss due to the mechanical medium resistance. We demonstrate that mechanical friction due to strong interactions, for example of quarks in quark-gluon plasma, can induce significant soft photon radiation.",2004.09634v2 2020-04-28,Temperature-Dependent Resistivity of Alternative Metal Thin Films,"The temperature coefficients of the resistivity (TCR) of Cu, Ru, Co, Ir, and W thin films have been investigated as a function of film thickness below 10 nm. Ru, Co, and Ir show bulk-like TCR values that are rather independent of the thickness whereas the TCR of Cu increases strongly with decreasing thickness. Thin W films show negative TCR values, which can be linked to high disorder. The results are qualitatively consistent with a temperature-dependent semiclassical thin film resistivity model that takes into account phonon, surface, and grain boundary scattering.",2004.13854v3 2007-10-26,Transport and magnetic properties in YBaCo2O5.45: Focus on the high-temperature transition,"The electronic transport properties and the magnetic susceptibility were measured in detail in $YBaCo_2O_{5.45}$. Close to the so-called metal-insulator transition, strong effects of resistance relaxation, a clear thermal hysteresis and a sudden increase of the resistance noise are observed. This is likely due to the first order character of the transition and to the underlying phases coexistence. Despite these out of equilibrium features, a positive and linear magneto-resistance is also observed, possibly linked to the heterogeneity of the state. From a magnetic point of view, the paramagnetic to ordered magnetic state transition is observed using non linear susceptibilty. This transition shows the characteristics of a continuous transition, and time dependent effects can be linked with the dynamics of magnetic domains in presence of disorder. Thus, when focusing on the order of the transitions, the electronic one and the magnetic one can not be directly associated.",0710.5008v1 2017-04-24,Near-perfect spin filtering and negative differential resistance in an Fe(II)S complex,"Density functional theory and nonequilibrium Green's function calculations have been used to explore spin-resolved transport through the high-spin state of an iron(II)sulfur single molecular magnet. Our results show that this molecule exhibits near-perfect spin filtering, where the spin-filtering efficiency is above 99%, as well as significant negative differential resistance centered at a low bias voltage. The rise in the spin-up conductivity up to the bias voltage of 0.4 V is dominated by a conductive lowest unoccupied molecular orbital, and this is accompanied by a slight increase in the magnetic moment of the Fe atom. The subsequent drop in the spin-up conductivity is because the conductive channel moves to the highest occupied molecular orbital which has a lower conductance contribution. This is accompanied by a drop in the magnetic moment of the Fe atom. These two exceptional properties, and the fact that the onset of negative differential resistance occurs at low bias voltage, suggests the potential of the molecule in nanoelectronic and nanospintronic applications.",1704.07327v1 2017-07-08,Electron and thermal transport via Variable Range Hopping in MoSe$_{2}$ single crystals,"Bulk single crystal Molybdenum diselenide has been studied for its electronic and thermal transport properties. We perform resistivity measurements with current in-plane (CIP) and current perpendicular to plane (CPP) as a function of temperature. The CIP measurements exhibit metal to semiconductor transition at $\simeq 31$ K. In the semiconducting phase ($T > 31$ K), the transport is best explained by variable range hopping (VRH) model. Large magnitude of resistivity in CPP mode indicates strong structural anisotropy. Seebeck coefficient as a function of temperature measured in the range $90 - 300$ K, also agrees well with the VRH model. The room temperature Seebeck coefficient is found to be $139$ $\mu$V/K. VRH fittings of the resistivity and Seebeck coefficient data indicate high degree of localization.",1707.02426v1 2015-04-14,Voltage equilibration for reactive atomistic simulations of electrochemical processes,"We introduce EChemDID, a model to describe electrochemical driving force in reactive molecular dynamics simulations. The method describes the equilibration of external electrochemical potentials (voltage) within metallic structures and their effect on the self consistent partial atomic charges used in reactive molecular dynamics. An additional variable assigned to each atom denotes the local potential in its vicinity and we use fictitious, but computationally convenient, dynamics to describe its equilibration within not-simply connected metallic structures on-the-fly during the molecular dynamics simulation. This local electrostatic potential is used to dynamically modify the atomic electronegativities used to compute partial atomic changes via charge equilibration. Validation tests show that the method provides an accurate description of the electric fields generated by the applied voltage and the driving force for electrochemical reactions. We demonstrate EChemDID via simulations of the operation of electrochemical metallization cells. The simulations predict the switching of the device between a high-resistance to a low-resistance state as a conductive metallic bridge is formed and resistive currents that can be compared with experimental measurements. In addition to applications in nanoelectronics, EChemDID could be useful to model electrochemical energy conversion devices.",1504.03621v1 2016-09-29,Magnetotransport properties and evidence of topological insulating state in LaSbTe,"In this report, we present the magnetotransport and magnetization properties of LaSbTe single crystals. Magnetic field-induced turn-on behavior and low-temperature resistivity plateau have been observed. By adopting both metal-semiconductor crossover and Kohler scaling analysis, we have discussed the possible origin of the temperature and magnetic field dependence of resistivity. At 5 K and 9 T, a large, non-saturating transverse magnetoresistance (MR) $\sim$ 5$\times$10$^{3}$ \% has been obtained. The MR shows considerable anisotropy, when the magnetic field is applied along different crystallographic directions. The non-linear field dependence of the Hall resistivity confirms the presence of two types of charge carriers. From the semiclassical two-band fitting of Hall conductivity and longitudinal conductivity, very high carrier mobilities and almost equal electron and hole densities have been deduced, which result in large MR. The Fermi surface properties have been analyzed from de Haas-van Alphen oscillation. From the magnetization measurement, the signature of non-trivial surface state has been detected, which confirms that LaSbTe is a topological insulator, consistent with the earlier first-principles calculations.",1609.09397v3 2019-11-20,Investigation of the phase separation property in La$_{0.2}$Pr$_{0.4}$Ca$_{0.4}$MnO$_3$ manganite,"We report a comprehensive investigation of La0.2Pr0.4Ca0.4MnO3 to clarify the micrometre scale phase separation phenomenon in the mixed valent manganite (La,Pr,Ca)MnO3. The compound shows multiple magnetic transitions, in which the charge-ordered state is converted into a ferromagnetic state in steps with the application of a magnetic field. The ac susceptibility measurements show that the glassy transition at low temperatures does not depend on the frequency, thus indicating the absence of any spin glass behaviour. Magnetization as well as heat capacity measurements indicate that this low temperature transition is magnetic field dependent. The field dependent resistivity at 2K shows a sharp drop indicating that the sample behaviour changes from a high resistive state to a low resistive state, corroborating the conversion of charge-ordered insulating (COI) phase to a ferromagnetic metallic (FMM) phase. Our results point towards the existence of phase separation, rigidity of the low temperature glassy-like phase as well as the conversion of COI phase to FMM phase by the application of magnetic fields.",1911.08881v1 2021-02-01,Real-time Hall-effect detection of current-induced magnetization dynamics in ferrimagnets,"Measurements of the transverse Hall resistance are widely used to investigate electron transport, magnetization phenomena, and topological quantum states. Owing to the difficulty of probing transient changes of the transverse resistance, the vast majority of Hall effect experiments are carried out in stationary conditions using either dc or ac currents. Here we present an approach to perform time-resolved measurements of the transient Hall resistance during current-pulse injection with sub-nanosecond temporal resolution. We apply this technique to investigate in real-time the magnetization reversal caused by spin-orbit torques in ferrimagnetic GdFeCo dots. Single-shot Hall effect measurements show that the current-induced switching of GdFeCo is widely distributed in time and characterized by significant activation delays, which limit the total switching speed despite the high domain-wall velocity typical of ferrimagnets. Our method applies to a broad range of current-induced phenomena and can be combined with non-electrical excitations to perform pump-probe Hall effect measurements.",2102.00716v1 2021-04-23,Deformation and tearing of graphene-reinforced elastomer nanocomposites,"The resistance to failure through tearing is a crucial mechanical property for the application of different elastomers. In this work, graphene nanoplatelets (GNPs) were introduced into a fluoroelastomer (FKM) matrix with the aim of improving its tear resistance. The fracture energy through tearing was evaluated using the pure shear test. It was found that the tearing energy increased linearly with the volume fraction of the GNPs. At the maximum GNP content, the tearing resistance was 3 times higher, suggesting efficient toughening from the GNPs. Theoretical analysis of the micromechanics was conducted by considering debonding and pull-out of the nanoplatelets as possible toughening mechanisms. It was determined quantitatively that the main toughening mechanism was debonding of the interface rather than pull-out. The formation of cavities at flake ends during the deformation, as confirmed by scanning electron microscopy, was found to contribute to the remarkably high interfacial debonding energy (~1 kJ/m2).",2104.11535v1 2021-04-27,Electronegative metal dopants improve switching consistency in Al2O3 resistive switching devices,"Resistive random access memories are promising for non-volatile memory and brain-inspired computing applications. High variability and low yield of these devices are key drawbacks hindering reliable training of physical neural networks. In this study, we show that doping an oxide electrolyte, Al2O3, with electronegative metals makes resistive switching significantly more reproducible, surpassing the reproducibility requirements for obtaining reliable hardware neuromorphic circuits. The underlying mechanism is the ease of creating oxygen vacancies in the vicinity of electronegative dopants, due to the capture of the associated electrons by dopant mid-gap states, and the weakening of Al-O bonds. These oxygen vacancies and vacancy clusters also bind significantly to the dopant, thereby serving as preferential sites and building blocks in the formation of conducting paths. We validate this theory experimentally by implanting multiple dopants over a range of electronegativities, and find superior repeatability and yield with highly electronegative metals, Au, Pt and Pd. These devices also exhibit a gradual SET transition, enabling multibit switching that is desirable for analog computing.",2104.13301v2 2021-05-06,Contact resistance of various metallisation schemes to superconducting boron doped diamond between 1.9 and 300 K,"Diamond is a material that offers potential in numerous device applications. In particular, highly boron doped diamond is attractive due to its superconductivity and high Young's Modulus. The fabrication of stable, low resistance, ohmic contacts is essential to ensure proper device function. Previous work has established the efficacy of several methods of forming suitable contacts to diamond at room temperature and above, including carbide forming and carbon soluble metallisation schemes. Herein, the stability of several contact schemes (Ti, Cr, Mo, Ta and Pd) to highly boron doped nanocrystalline diamond was verified down to the cryogenic temperatures with modified Transmission Line Model (TLM) measurements. While all contact schemes remained ohmic, a significant temperature dependency is noted at Tc and at the lowest temperatures the contact resistances ranged from Ti/Pt/Au with ${(8.83 \pm 0.10)\times 10^{-4} \:{\Omega}.cm}$ to Ta/Pt/Au with ${(8.07 \pm 0.62) \times 10^{-6} \:{\Omega}.cm}$.",2105.02839v1 2021-08-10,Giant Piezospintronic Effect in a Noncollinear Antiferromagnetic Metal,"One of the main bottleneck issues for room-temperature antiferromagnetic spintronic devices is the small signal read-out owing to the limited anisotropic magnetoresistance in antiferromagnets. However, this could be overcome by either utilizing the Berry-curvature-induced anomalous Hall resistance in noncollinear antiferromagnets or establishing tunnel junction devices based on effective manipulation of antiferromagnetic spins. In this work, we demonstrate the giant piezoelectric strain control of the spin structure and the anomalous Hall resistance in a noncollinear antiferromagnetic metal - D019 hexagonal Mn3Ga. Furthermore, we built tunnel junction devices with a diameter of 200 nm to amplify the maximum tunneling resistance ratio to more than 10% at room-temperature, which thus implies significant potential of noncollinear antiferromagnets for large signal-output and high-density antiferromagnetic spintronic device applications.",2108.04439v1 2021-09-07,Strain-dependent resistance and giant gauge factor in monolayer WSe2,"We report the strong dependence of resistance on uniaxial strain in monolayer WSe2 at various temperatures, where the gauge factor can reach as large as 2400. The observation of strain-dependent resistance and giant gauge factor is attributed to the emergence of nonzero Berry curvature dipole. Upon increasing strain, Berry curvature dipole can generate net orbital magnetization, which would introduce additional magnetic scattering, decreasing the mobility and thus conductivity. Our work demonstrates the strain engineering of Berry curvature and thus the transport properties, making monolayer WSe2 potential for the application in the high-performance flexible and transparent electronics.",2109.02980v1 2021-09-12,Coexistence of resistance oscillations and the anomalous metal phase in a lithium intercalated TiSe$_2$ superconductor,"Superconductivity and charge density wave (CDW) appear in the phase diagram of a variety of materials including the high - $T$$_c$ cuprate family and many transition metal dichalcogenides (TMDs). Their interplay may give rise to exotic quantum phenomena. Here, we show that superconducting arrays can spontaneously form in TiSe$_2$ - a TMD with coexisting superconductivity and CDW - after lithium ion intercalation. We induce a superconducting dome in the phase diagram of Li$_x$TiSe$_2$ by using the ionic solid-state gating technique. Around optimal doping, we observe magnetoresistance oscillations, indicating the emergence of periodically arranged domains. In the same temperature, magnetic field and carrier density regime where the resistance oscillations occur, we observe signatures for the anomalous metal - a state with a resistance plateau across a wide temperature range below the superconducting transition. Our study not only sheds further insight into the mechanism for the periodic electronic structure, but also reveals the interplay between the anomalous metal and superconducting fluctuations.",2109.05450v1 2021-10-11,Observation of Exchange Bias in Antiferromagnetic Cr$_{0.79}$Se due to the Coexistence of Itinerant Weak Ferromagnetism at Low-temperatures,"We report on the structural, electrical transport, and magnetic properties of antiferromagnetic transition-metal monochalcogenide Cr$_{0.79}$Se. Different from the existing off-stoichiometric compositions, Cr$_{0.79}$Se is found to be synthesised into the same NiAs-type hexagonal crystal structure of CrSe. Resistivity data suggest Cr$_{0.79}$Se to be a Fermi-liquid-type metal at low temperatures, while at intermediate temperatures the resistivity depends sublinearly on the temperature. Eventually, at the elevated temperatures the rate of change of resistivity rapidly decreases with increasing temperature. Magnetic measurements suggest a transition from paramagnetic phase to an antiferromagnetic phase at a N$\acute{e}$el temperature of 225 K. Further reduction of the sample temperature results into coexistance of weak ferromagnetism along with the antiferromagnetic phase below 100 K. As a result, below 100 K, we identify significant exchange bias due to the interaction between the ferro- and antiferromagnetic phases. In addition, from the temperature dependent X-ray diffraction measurements we observe that the NiAs-type structure is stable up to as high as 600$^o$C.",2110.05058v1 2022-06-16,Fill Factor Losses and Deviations from the Superposition Principle in Lead-Halide Perovskite Solar Cells,"The enhancement of the fill factor in the current generation of perovskite solar cells is the key for further efficiency improvement. Thus, methods to quantify the fill factor losses are urgently needed. A classical method to quantify Ohmic and non-Ohmic resistive losses in solar cells is based on the comparison between the voltage in the dark and under illumination analysed at equal recombination current density. Applied to perovskite solar cells, we observe a combination of an Ohmic series resistance with a voltage-dependent resistance that is most prominent at short circuit and low forward bias. The latter is most likely caused by the poor transport properties of the electron and/or hole transport layers. By measuring the photoluminescence of perovskite solar cells as a function of applied voltage, we provide direct evidence for a high quasi-Fermi level splitting at low and moderate forward bias that substantially exceeds the externally applied voltage. This quasi-Fermi level splitting causes recombination losses and, thus, reduces both the short-circuit current and the fill factor of the solar cell.",2207.02297v1 2022-12-07,Self-assembled neuromorphic networks at self-organized criticality in Ag-hBN platform,"Networks and systems which exhibit brain-like behavior can analyze information from intrinsically noisy and unstructured data with very low power consumption. Such characteristics arise due to the critical nature and complex interconnectivity of the brain and its neuronal network. We demonstrate that a system comprising of multilayer hexagonal Boron Nitride (hBN) films contacted with Silver (Ag), that can uniquely host two different self-assembled networks, which are self-organized at criticality (SOC). This system shows bipolar resistive switching between high resistance (HRS) and low resistance states (LRS). In the HRS, Ag clusters (nodes) intercalate in the van der Waals gaps of hBN forming a network of tunnel junctions, whereas the LRS contains a network of Ag filaments. The temporal avalanche dynamics in both these states exhibit power-law scaling, long-range temporal correlation, and SOC. These networks can be tuned from one to another with voltage as a control parameter. For the first time, different neuron-like networks are realized in a single CMOS compatible, 2D materials platform.",2301.01619v1 2023-06-13,An Evaluation of Multi-Component Weft-Knitted Twill Structures for Sensing Tensile Force,"We present multi-component knitted resistive sensors for tracking tensile force. The knits were fabricated using a Twill structure, which is a simple pattern featuring anisotropic elastic behavior, providing high stability along course-direction. Our sensors are made of two commercially available conductive yarn types, with highly different linear resistance. We present a variety of integration methods using the proposed Twill structure, all of which can be easily replicated on a two-bed weft-knitting machine. We evaluate the performance of the resulting sensor variations, with respect to consistency, hysteresis, short-term and long-term relaxation and drift, among other metrics. We found that particulars of the knit's loop composition have a crucial effect on the consistency of the sensor readings. Furthermore, we show that knitting resistive yarn more tightly than the substrate material gives superior results and that improving elastic recoil by adding Lycra to the supporting substrate can considerably improve performance.",2306.07612v1 2024-04-13,Combinatorial Printing of Functionally Graded Solid-State Electrolyte for High-Voltage Lithium Metal Batteries,"Heterogeneous multilayered solid-state electrolyte (HMSSE) has been widely explored for their broadened working voltage range and compatibility with electrodes. However, due to the limitations of traditional manufacturing methods such as casting, the interface between electrolyte layers in HMSSE can decrease the ionic conductivity severely. Here, a novel combinatory aerosol jet printing (CAJP) is introduced to fabricate functionally graded solid-state electrolyte (FGSSE) without sharp interface. Owing to the unique ability of CAJP (in-situ mixing and instantaneous tuning of the mixing ratio), FGSSE with smooth microscale compositional gradation is achieved. Electrochemical tests show that FGSSE has excellent oxidative stability exceeding 5.5 V and improved conductivity (>7 times of an analogous HMSSE). By decoupling the total resistance, we show that the resistance from the electrolyte/electrolyte interface of HMSSE is 5.7 times of the total resistance of FGSSE. The Li/FGSSE/NCM622 cell can be stably run for more than 200 cycles along with improved rate performance.",2404.09008v1 2024-05-29,Multipacting mitigation by atomic layer deposition: the case study of Titanium Nitride,"This study investigates the use of Atomic Layer deposition (ALD) to mitigate multipacting phenomena inside superconducting radio frequency (SRF) cavities used in particle accelerators. The unique ALD capability to control the film thickness down to the atomic level on arbitrary complex shape objects enable the fine tuning of TiN film resistivity and total electron emission yield (TEEY) from coupons to devices. This level of control allows us to adequately choose a TiN film thickness that provide both a high resistivity to prevent Ohmic losses and low TEEY to mitigate multipacting for the application of interest. The methodology presented in this work can be scaled to other domain and devices subject to RF fields in vacuum and sensitive to multipacting or electron discharge processes with their own requirements in resistivities and TEEY values",2405.18949v1 2015-05-29,Few Layer HfS2 FET,"2D materials are expected to be favorable channel materials for field-effect transistor (FET) with extremely short channel length because of their superior immunity to short-channel effects (SCE). Graphene, which is the most famous 2D material, has no bandgap without additional techniques and this property is major hindrance in reducing the drain leakage. Therefore, 2D materials with finite band gap, such as transition metal dichalcogenides (TMDs, e.g. MoS2 WSe2) or phosphorene, are required for the low power consumption FETs. Hafnium disulfide (HfS2) is a novel TMD, which has not been investigated as channel material. We focused on its potential for well-balanced mobility and bandgap properties. The higher electron affinity of Hf dichalcogenides compared with Mo or W chalcogenides facilitates the formation of low resistance contact and staggered heterojunction with other 2D materials. Here we demonstrate the first few layer HfS2 FET with robust current saturation and high current on/off ratio of more than 10^4.",1505.07970v1 2011-10-29,From mixed valence to the Kondo lattice regime,"Many heavy fermion materials are known to crossover from the Kondo lattice regime to the mixed-valent regime or vice-versa as a function of pressure or doping. We study this crossover theoretically by employing the periodic Anderson model within the framework of the dynamical mean field theory. Changes occurring in the dynamics and transport across this crossover are highlighted. As the valence is decreased (increased) relative to the Kondo lattice regime, the Kondo resonance broadens significantly, while the lower (upper) Hubbard band moves closer to the Fermi level. The resistivity develops a two peak structure in the mixed valent regime: a low temperature coherence peak and a high temperature 'Hubbard band' peak. These two peaks merge yielding a broad shallow maximum upon decreasing the valence further. The optical conductivity, likewise exhibits an unusual absorption feature (shoulder) in the deep mid-infrared region, which grows in intensity with decreasing valence. The involvement of the Hubbard bands in dc transport, and of the effective f-level in the optical conductivity are shown to be responsible for the anomalous transport properties. A two-band hybridization-gap model, which neglects incoherent effects due to many-body scattering, commonly employed to understand the optical response in these materials is shown to be inadequate, especially in the mixed-valent regime. Comparison of theory with experiment carried out for (a) dc resistivities of CeRhIn5, Ce2Ni3Si5, CeFeGe3 and YbIr2Si2; (b) pressure dependent resistivity of YbInAu2 and CeCu6; and (c) optical conductivity measurements in YbIr2Si2 yields excellent agreement.",1110.6498v1 2021-04-01,Enhanced spin injection in molecularly functionalized graphene via ultra-thin oxide barriers,"Realisation of practical spintronic devices relies on the ability to create and detect pure spin currents. In graphene-based spin valves this is usually achieved by injection of spin-polarized electrons from ferromagnetic contacts via a tunnel barrier, with Al2O3 and MgO used most widely as barrier materials. However, the requirement to make these barriers sufficiently thin often leads to pinholes and low contact resistances which in turn results in low spin injection efficiencies, typically 5% at room temperature, due to the so-called resistance mismatch problem. Here we demonstrate an alternative approach to fabricate ultra-thin tunnel barrier contacts to graphene. We show that laser-assisted chemical functionalization of graphene with sp3-bonded phenyl groups effectively provides a seed layer for growth of ultrathin Al2O3 films, ensuring smooth, high quality tunnel barriers and an enhanced spin injection efficiency. Importantly, the effect of functionalization on spin transport in the graphene channel itself is relatively weak, so that the enhanced spin injection dominates and leads to an order of magnitude increase in spin signals. Furthermore, spatial control of functionalization using a focused laser beam and lithographic techniques can in principle be used to limit functionalization to contact areas only, further reducing the effect on the graphene channel. Our results open a new route towards circumventing the resistance mismatch problem in graphene-based spintronic devices based on the easily available and highly stable Al2O3, and facilitate a step forward in the development of their practical applications.",2104.00709v1 2017-05-16,Application of flash method in the measurements of interfacial thermal resistance in layered and particulate composite materials,"Presented study concerns the possibility of evaluation of interfacial thermal resistance (ITR) between the constituents in composite materials with the use of flash technique. Two variants of such measurement are considered, the first of which is the measurement of ITR between two bonded layers of different materials which had been studied before by various researchers. The second tested measurement method is targeted at determination of ITR in particulate composites with low and moderate filler content based on their effective thermal conductivity. Method of such measurement is proposed and tested on two cases of particle-filled polymer composites. Positive verification results were obtained for polymer/glass composite in which the difference between thermal conductivities of matrix and filler is low. For a polymer filled with aluminum particles the evaluation of average ITR in the samples was impossible as the effective medium models applied in the method strongly underestimated the thermal conductivity of that material. The investigation confirmed the need for more accurate methods of macroscopic thermal properties prediction for composite media with high contrast of thermal conductivities of the constituents. Extended literature study suggests that the method can be applicable to selected classes of engineering materials.",1705.05621v1 1998-12-23,Temperature dependence of electric resistance and magnetoresistance of pressed nanocomposites of multilayer nanotubes with the structure of nested cones,"Bulk samples of carbon multilayer nanotubes with the structure of nested cones (fishbone structure) suitable for transport measurements, were prepared by compressing under high pressure (~25 kbar) a nanotube precursor synthesized through thermal decomposition of polyethylene catalyzed by nickel. The structure of the initial nanotube material was studied using high-resolution transmission electron microscopy. In the low-temperature range (4.2 - 100 K) the electric resistance of the samples changes according to the law ln \rho ~ (T_0/T)^{1/3}, where T_0 ~ 7 K. The measured magnetoresistance is quadratic in the magnetic field and linear in the reciprocal temperature. The measurements have been interpreted in terms of two-dimensional variable-range hopping conductivity. It is suggested that the space between the inside and outside walls of nanotubes acts as a two-dimensional conducting medium. Estimates suggest a high value of the density of electron states at the Fermi level of about 5 10^{21} eV^{-1} cm^{-3}.",9812384v1 2017-01-07,"Spatially uniform resistance switching of low current, high endurance titanium-niobium-oxide memristors","We analyzed micrometer-scale titanium-niobium-oxide prototype memristors, which exhibited low write-power (<3 {\mu}W) and energy (<200 fJ/bit/{\mu}m2), low read-power (~nW), and high endurance (>millions of cycles). To understand their physico-chemical operating mechanisms, we performed in-operando synchrotron x-ray transmission nanoscale spectromicroscopy using an ultra-sensitive time-multiplexed technique. We observed only spatially uniform material changes during cell operation, in sharp contrast to the frequently detected formation of a localized conduction channel in transition-metal-oxide memristors. We also associated the response of assigned spectral features distinctly to non-volatile storage (resistance change) and writing of information (application of voltage and Joule heating). These results provide critical insights into high-performance memristors that will aid in device design, scaling and predictive circuit-modeling, all of which are essential for the widespread deployment of successful memristor applications.",1701.01784v1 2001-02-09,Superconducting Properties of MgB2 Bulk Materials Prepared by High Pressure Sintering,"High-density bulk materials of a newly discovered 40K intermetallic MgB2 superconductor were prepared by high pressure sintering. Superconducting transition with the onset temperature of 39K was confirmed by both magnetic and resistive measurements. Magnetization versus field (M-H) curve shows the behavior of a typical Type II superconductor and the lower critical field Hc1(0) estimated from M-H curve is 0.032T. The bulk sample shows good connection between grains and critical current density Jc estimated from the magnetization hysteresis using sample size was 2x104A/cm2 at 20K and 1T. Upper critical field Hc2(0) determined by extrapolating the onset of resistive transition and assuming a dirty limit is 18T.",0102167v1 2018-09-17,High quality factor graphene-based 2D heterostructure mechanical resonator,"Ultralight mechanical resonators based on low-dimensional materials are well suited as exceptional transducers of minuscule forces or mass changes. However, the low dimensionality also provides a challenge to minimize resistive losses and heating. Here, we report on a novel approach that aims to combine different 2D materials to tackle this challenge. We fabricated a heterostructure mechanical resonator consisting of few layers of niobium diselenide (NbSe$_2$) encapsulated by two graphene sheets. The hybrid membrane shows high quality factors up to 245'000 at low temperatures, comparable to the best few-layer graphene mechanical resonators. In contrast to few-layer graphene resonators, the device shows reduced electrical losses attributed to the lower resistivity of the NbSe$_2$ layer. The peculiar low temperature dependence of the intrinsic quality factor points to dissipation over two-level systems which in turn relax over the electronic system. Our high sensitivity readout is enabled by coupling the membrane to a superconducting cavity which allows for the integration of the hybrid mechanical resonator as a sensitive and low loss transducer in future quantum circuits.",1809.06169v1 2022-04-22,Comparison of different sensor thicknesses and substrate materials for the monolithic small collection-electrode technology demonstrator CLICTD,"Small collection-electrode monolithic CMOS sensors profit from a high signal-to-noise ratio and a small power consumption, but have a limited active sensor volume due to the fabrication process based on thin high-resistivity epitaxial layers. In this paper, the active sensor depth is investigated in the monolithic small collection-electrode technology demonstrator CLICTD. Charged particle beams are used to study the charge-collection properties and the performance of devices with different thicknesses both for perpendicular and inclined particle incidence. In CMOS sensors with a high-resistivity Czochralski substrate, the depth of the sensitive volume is found to increase by a factor two in comparison with standard epitaxial material and leads to significant improvements in the hit-detection efficiency and the spatial and time resolution.",2204.10569v2 2021-11-01,A New Class of Alumina-Forming Superalloy for 3D Printing,"A new class of crack-resistant nickel-based superalloy containing high $\gamma^\prime$ fraction is studied for the laser-powder bed fusion (L-PBF) process. The effects of the (Nb+Ta)/Al ratio is emphasised, a strategy that is shown to confer excellent low-temperature strength whilst maintaining oxidation resistance at high temperatures via stable alumina scale formation. The processability of the new alloys is characterised with respect to defect assessment by micro-focus x-ray computed tomography; use is made of a prototype turbine blade geometry and the heritage alloy CM247LC as a benchmark. In all cases, some processing-related porosity is present in thin wall sections such as the trailing edge, but this can be avoided by judicious processing. The cracking seen in CM247LC -- in solid-state, liquation and solidification forms -- is avoided. A novel sub-solvus heat treatment strategy is proposed which takes advantage of AM not requiring solutioning; super-solvus heat treatment is inappropriate since it embrittles the material by deterioration of the texture and coarsening of grain boundary carbides. The tensile strength of the new superalloy is greatest when the Nb+Ta content is highest and exceeds that of CM247LC up to $\sim$900$\,$$^\circ$C. The oxidation resistance is best when Al content is highest, and oxidation-assisted cracking resistance maximized when the (Nb+Ta)/Al ratio is balanced. In all cases these are equivalent or superior to that of CM247LC. Nevertheless, the creep resistance of the new alloys is somewhat inferior to that of CM247LC for which the $\gamma^\prime$, C, and B contents are higher; this implies a processing/property trade-off which requires further clarification.",2111.01049v1 2005-11-08,Development of the Charge Particle Detector Based on CVD - Diamond,"High radiation hardness, chemical resistance, high temperature operation capabilities stimulate a growing interest to use diamond materials as detectors of ionizing radiation. Samples of CVD-diamond materials in sizes 12 square mm and 4 square mm with thickness from 50 microns up to 500 microns have been grown in INR RAS using a DC glow discharge in a mixture of gases CH4/H2 on molybdenum substrates.",0511068v1 2018-10-24,High Strain Rate Behaviour of Nano-quasicrystalline Al93Fe3Cr2Ti2 Alloy and Composites,"In the present work, we demonstrate for the first time the outstanding dynamic mechanical properties of nano-quasicrystalline Al93Fe3Cr2Ti2 at.% alloy and composites. Unlike most crystalline aluminium-based alloys, this alloy and composites exhibit substantial strain rate sensitivity and retain much of their ductility at high rates of strain. This opens new pathways for use in safety-critical materials where impact resistance is required.",1810.10476v2 2019-12-24,Large spin Hall angle and spin mixing conductance in highly resistive antiferromagnetic Mn2Au,"Antiferromagnetic (AFM) materials recently have shown interest in the research in spintronics due to its zero stray magnetic field, high anisotropy, and spin orbit coupling. In this context, the bi-metallic AFM Mn2Au has drawn attention because it exhibits unique properties and its Neel temperature is very high. Here, we report spin pumping and inverse spin Hall effect investigations in Mn2Au and CoFeB bilayer system using ferromagnetic resonance. We found large spin Hall angle {\theta}_SH = 0.22",1912.11522v2 2008-09-09,Printed Graphene Circuits,"we have fabricated transparent electronic devices based on graphene materials with thickness down to one single atomic layer by the transfer printing method. The resulting printed graphene devices retain high field effect mobility and have low contact resistance. The results show that the transfer printing method is capable of high-quality transfer of graphene materials from silicon dioxide substrates, and the method thus will have wide applications in manipulating and delivering graphene materials to desired substrate and device geometries. Since the method is purely additive, it exposes graphene (or other functional materials) to no chemical preparation or lithographic steps, providing greater experimental control over device environment for reproducibility and for studies of fundamental transport mechanisms. Finally, the transport properties of the graphene devices on the PET substrate demonstrate the non-universality of minimum conductivity and the incompleteness of the current transport theory.",0809.1634v1 2021-08-29,A graph based workflow for extracting grain-scale toughness from meso-scale experiments,"We introduce a novel machine learning computational framework that aims to compute the material toughness, after subjected to a short training process on a limited meso-scale experimental dataset. The three part computational framework relies on the ability of a graph neural network to perform high accuracy predictions of the micro-scale material toughness, utilizing a limited size dataset that can be obtained from meso-scale fracture experiments. We analyze the functionality of the different components of the framework, but the focus is on the capabilities of the neural network. The minimum size of the dataset required for the network training is investigated. The results demonstrate the high efficiency of the algorithm in predicting the crack growth resistance in micro-scale level, using a crack path trajectory limited to 200-300 grains for the network training. The merit of the proposed framework arises from the capacity to enhance its performance in different material systems with a limited additional training on data obtained from experiments that do not require complex or cumbersome measurements. The main objective is the development of an efficient computational tool that enables the study of a wide range of material microstructure properties and the investigation of their influence on the material toughness.",2108.12783v1 2022-08-25,Magnetoresistive behaviour of ternary Cu-based materials processed by high-pressure torsion,"Severe plastic deformation using high-pressure torsion of ternary Cu-based materials (CuFeCo and CuFeNi) was used to fabricate bulk samples with a nanocrystalline microstructure. The goal was to produce materials featuring the granular giant magnetoresistance effect, requiring interfaces between ferro- and nonmagnetic materials. This magnetic effect was found for both ternary systems; adequate subsequent annealing had a positive influence. The as-deformed states, as well as microstructural changes upon thermal treatments, were studied using scanning electron microscopy and X-ray diffraction measurements. Deducing from electron microscopy, a single-phase structure was observed for all as-deformed samples, indicating the formation of a supersaturated solid solution. However, judging from the presence of the granular giant-magnetoresistive effect, small ferromagnetic particles have to be present. The highest drop in room temperature resistivity (2.45% at 1790 kA/m) was found in Cu62Fe19Ni19 after annealing for 1 h at 400 {\deg}C. Combining the results of classical microstructural studies and magnetic measurements, insights into the evolution of ferromagnetic particles are accessible.",2208.11895v1 2023-03-28,Electrolyte Coatings for High Adhesion Interfaces in Solid-state Batteries from First Principles,"We introduce an adhesion parameter that enables rapid screening for materials interfaces with high adhesion. This parameter is obtained by density functional theory calculations of individual single-material slabs rather than slabs consisting of combinations of two materials, eliminating the need to calculate all configurations of a prohibitively vast space of possible interface configurations. Cleavage energy calculations are used as an upper bound for electrolyte and coating energies and implemented in an adapted contact angle equation to derive the adhesion parameter. In addition to good adhesion, we impose further constraints in electrochemical stability window, abundance, bulk reactivity, and stability to screen for coating materials for next-generation solid-state batteries. Good adhesion is critical in combating delamination and resistance to Lithium diffusivity in solid-state batteries. Here, we identify several promising coating candidates for the Li7La3Zr2O12 and sulfide electrolyte systems including the previously investigated electrode coating materials LiAlSiO4 and Li5AlO8, making them especially attractive for experimental optimization and commercialization.",2303.16350v1 2014-12-12,High-T_c superconductivity in ultrathin Bi_2Sr_2CaCu_2O_8+x down to halfunit-cell thickness by protection with graphene,"High-T_c superconductors confined to two dimension exhibit novel physical phenomena, such as superconductor-insulator transition. In the Bi_2Sr_2CaCu_2O_8+x (Bi2212) model system, despite extensive studies, the intrinsic superconducting properties at the thinness limit have been difficult to determine. Here we report a method to fabricate high quality single-crystal Bi2212 films down to half-unit-cell thickness in the form of graphene/Bi2212 van der Waals heterostructure, in which sharp superconducting transitions are observed. The heterostructure also exhibits a nonlinear current-voltage characteristic due to the Dirac nature of the graphene band structure. More interestingly, although the critical temperature remains essentially the same with reduced thickness of Bi2212, the slope of the normal state T-linear resistivity varies by a factor of 4-5, and the sheet resistance increases by three orders of magnitude, indicating a surprising decoupling of the normal state resistance and superconductivity. The developed technique is versatile, applicable to investigate other two-dimensional (2D) superconducting materials.",1412.3896v1 2019-08-18,Maximizing the spin-orbit torque efficiency of Pt/Ti multilayers by optimization of the tradeoff between the intrinsic spin Hall conductivity and carrier lifetime,"We report a comprehensive study of the maximization of the spin Hall ratio ({\theta}SH) in Pt thin films by the insertion of sub-monolayer layers of Ti to decrease carrier lifetime while minimizing the concurrent reduction in the spin Hall conductivity. We establish that the intrinsic spin Hall conductivity of Pt, while robust against the strain and the moderate interruption of crystal order caused by these insertions, begins to decrease rapidly at high resistivity level because of the shortening carrier lifetime. The unavoidable trade-off between the intrinsic spin Hall conductivity and carrier lifetime sets a practical upper bound of {\theta}SH >=0.8 for heterogeneous materials where the crystalline Pt component is the source of the spin Hall effect and the resistivity is increased by shortening carrier lifetime. This work also establishes a very promising spin-Hall metal of [Pt 0.75 nm/Ti 0.2 nm]7/Pt 0.75 nm for energy-efficient, high-endurance spin-orbit torque technologies (e.g., memories, oscillators, and logic) due to its combination of a giant {\theta}SH of 0.8, or equivalently a dampinglike spin torque efficiency per unit current density of 0.35, with a relatively low resistivity (90 uOhm cm) and high suitability for practical technology integration.",1908.06528v1 2019-10-22,Transverse Beam Stability with Low-Impedance Collimators in the High Luminosity Large Hadron Collider: Status and Challenges,"The High-Luminosity upgrade of the Large Hadron Collider (HL-LHC) will double its beam intensity for the needs of High Energy Physics frontier. In order to ensure coherent stability until the beams are put in collision, the transverse impedance has to be reduced. As the major portion of the ring impedance is supplied by its collimation system, several low resistivity jaw materials have been proposed to lower the collimator impedance and a special collimator has been built and installed in the machine to study their effect. The results show a significant reduction of the resistive wall tune shift with novel materials, in agreement with the impedance model and the bench impedance and resistivity measurements. The largest improvement is obtained with a 5 {\mu}m Molybdenum coating of a Molybdenum-Graphite jaw. This coating can lower the machine impedance by up to 30% and the stabilizing Landau octupole threshold by up to 120 A. The collimators to be upgraded have been chosen based on the improvement of the octupole threshold, as well as the tolerance to steady state losses and failure scenarios. A half of the overall improvement can be obtained by coating the jaws of a subset of 4 out of 11 collimators identified as the highest contributors to machine impedance. This subset of low-impedance collimators is being installed during the Long Shutdown 2 in 2019-2020.",1910.09974v2 2020-11-05,Preparation of the AlTiNiCuCox system high-entropy alloys and structural analysis,"This study aimed to explore and develop a new material with high cost-effectiveness, excellent strength, light weight, high hardness, great wear resistance, corrosion resistance, and favorable oxidation resistance. Structural analysis suggested that, with the change in Co addition amount, the surface morphology and structure of the alloy system changed. XRD analysis indicated that, the alloy system was the FCC+BCC mixed structure. In addition, metallographical demonstrated that, with the increase in Co content, the dendritic crystal transformed from big block to dendritic structure, then to snowflake, gradually to petal-like, and finally to petal shape. SEM-EDS analysis revealed that, Cu element was enriched in interdendritic site, while Ti, Ni, Al and Co elements were enriched in dendrite. Besides, TEM and TEM-EDS analysis indicated that, there was nano-size precipitate of small particles in the Cu-enriched block region, along with dislocation; further, there was twin structure inside the dendrite, as well as the second phase with different morphology, and the second phase showed coherency with the matrix. The above analysis suggested that, the intercrystalline structure was the Cu-enriched phase of FCC structure; the internal matrix of grain was the NiTi and TiCo phases of BCC structure; and the second phases inside the grain were the AlCu2Ti,AlNi2Ti,AlCo2Ti and CuNi phases of FCC structure. Taken together, the AlTiNiCuCox system novel alloys have changed phase structures and phase types of the alloy system.",2011.02799v1 2022-01-19,Secondary Phase Limited Metal-Insulator Phase Transition in Chromium Nitride Thin Films,"Chromium nitride (CrN) is a well-known hard coating material that has found applications in abrasion and wear-resistant cutting tools, bearings, and tribology applications due to its high hardness, high-temperature stability, and corrosion-resistant properties. In recent years, CrN has also attracted significant interest due to its high thermoelectric power factor, and for its unique and intriguing metal-insulator phase transition. While CrN bulk single-crystals exhibit the characteristic metal-insulator transition accompanied with structural (orthorhombic-to-rocksalt) and magnetic (antiferromagnetic-to-paramagnetic) transition at ~260-280K, observation of such phase transition in thin-film CrN has been scarce and highly debated. In this work, the formation of the secondary metallic Cr2N phase during the growth is demonstrated to inhibit the observation of metal-insulator phase transition in CrN thin films. When the Cr-flux during deposition is reduced below a critical limit, epitaxial and stoichiometric CrN thin film is obtained that reproducibly exhibits the phase transition. Annealing of the mixed-phase film inside reducing NH3 environment converts the Cr2N into CrN, and a discontinuity in the electrical resistivity at ~ 277 K appears which supports the underlying hypothesis. A clear demonstration of the origin behind the controversy of the metal-insulator transition in CrN thin films marks significant progress and would enable its nanoscale device realization.",2201.07442v1 2022-01-22,High-throughput calculations combining machine learning to investigate the corrosion properties of binary Mg alloys,"Magnesium (Mg) alloys have shown great prospects as both structural and biomedical materials, while poor corrosion resistance limits their further application. In this work, to avoid the time-consuming and laborious experiment trial, a high-throughput computational strategy based on first-principles calculations is designed for screening corrosion-resistant binary Mg alloy with intermetallics, from both the thermodynamic and kinetic perspectives. The stable binary Mg intermetallics with low equilibrium potential difference with respect to the Mg matrix are firstly identified. Then, the hydrogen adsorption energies on the surfaces of these Mg intermetallics are calculated, and the corrosion exchange current density is further calculated by a hydrogen evolution reaction (HER) kinetic model. Several intermetallics, e.g. Y3Mg, Y2Mg and La5Mg, are identified to be promising intermetallics which might effectively hinder the cathodic HER. Furthermore, machine learning (ML) models are developed to predict Mg intermetallics with proper hydrogen adsorption energy employing work function (W_f) and weighted first ionization energy (WFIE). The generalization of the ML models is tested on five new binary Mg intermetallics with the average root mean square error (RMSE) of 0.11 eV. This study not only predicts some promising binary Mg intermetallics which may suppress the galvanic corrosion, but also provides a high-throughput screening strategy and ML models for the design of corrosion-resistant alloy, which can be extended to ternary Mg alloys or other alloy systems.",2201.09059v1 2019-10-17,High electrical conductivity in the epitaxial polar metals LaAuGe and LaPtSb,"Polar metals are an intriguing class of materials that simultaneously host free carriers and polar structural distortions. Despite the name ""polar metal,"" however, most well-studied polar metals are poor electrical conductors. Here, we demonstrate the molecular beam epitaxial (MBE) growth of LaPtSb and LaAuGe, two polar metal compounds whose electrical resistivity is an order of magnitude lower than the well studied oxide polar metals. These materials belong to a broad family of $ABC$ intermetallics adopting the stuffed wurtzite structure, also known as hexagonal Heusler compounds. Scanning transmission electron microscopy (STEM) reveals a polar structure with unidirectionally buckled $BC$ (PtSb, AuGe) planes. Magnetotransport measurements demonstrate good metallic behavior with low residual resistivity ($\rho_{LaAuGe}=59.05$ $\mu\Omega\cdot$cm and $\rho_{LaAPtSb}=27.81$ $\mu\Omega\cdot$cm at 2K) and high carrier density ($n_h\sim 10^{21}$ cm$^{-3}$). Photoemission spectroscopy measurements confirm the band metallicity and are in quantitative agreement with density functional theory (DFT) calculations. Through DFT-Chemical Pressure and Crystal Orbital Hamilton Population analyses, the atomic packing factor is found to support the polar buckling of the structure, though the degree of direct interlayer $B-C$ bonding is limited by repulsion at the $A-C$ contacts. When combined with insulating hexagonal Heuslers, these materials provide a new platform for fully epitaxial, multiferroic heterostructures.",1910.07685v1 2024-02-06,Physics-based Modeling of Pulse and Relaxation of High-rate Li/CF$_{x}$-SVO batteries in Implantable Medical Devices,"We present a physics-based model that accurately predicts the performance of Medtronic's implantable medical device battery lithium/carbon monofluoride (CF$_x$) - silver vanadium oxide (SVO) under both low-rate background monitoring and high-rate pulsing currents. The distinct properties of multiple active materials are reflected by parameterizing their thermodynamics, kinetics, and mass transport properties separately. Diffusion limitations of Li$^+$ in SVO are used to explain cell voltage transient behavior during pulse and post-pulse relaxation. We also introduce change in cathode electronic conductivity, Li metal anode surface morphology, and film resistance buildup to capture evolution of cell internal resistance throughout multi-year electrical tests. We share our insights on how the Li$^+$ redistribution process between active materials can restore pulse capability of the hybrid electrode, allow CF$_x$ to indirectly contribute to capacity release during pulsing, and affect the operation protocols and design principles of batteries with other hybrid electrodes. We also discuss additional complexities in porous electrode model parameterization and electrochemical characterization techniques due to parallel reactions and solid diffusion pathways across active materials. We hope our models implemented in the Hybrid Multiphase Porous Electrode Theory (Hybrid-MPET) framework can complement future experimental research and accelerate development of multi-active material electrodes with targeted performance.",2402.03677v1 2020-04-25,Reconciliation of experiments and theory on transport properties of iron and the geodynamo,"The amount of heat transport from the core, which constrains the dynamics and thermal evolution of the region, depends on the transport properties of iron. Ohta et al.(2016) and Konopkova et al.(2016) measured electrical resistivity and thermal conductivity of iron, respectively, in laser-heated diamond anvil cells (DACs) at relevant Earth's core pressure-temperature (P-T) conditions, and obtained dramatically contradictory results. Here we measure the electrical resistivity of hcp-iron up to ~170 GPa and ~3,000 K using a four-probe van der Pauw method coupled with homogeneous flat-top laser-heating in a DAC. We also compute its electrical and thermal conductivity by first-principles methods including electron-phonon and electron-electron scattering. We find that the measured resistivity of hcp-iron increases almost linearly with increasing temperature, and is consistent with current first-principles computations. The proportionality coefficient between resistivity and thermal conductivity (the Lorenz number) in hcp-iron differs from the ideal value (2.44*10^-8 W Omega K^-2), so a non-ideal Lorenz number of ~(2.0-2.1)*10^-8 W Omega K^-2 is used to convert the experimental resistivity to the thermal conductivity of hcp-Fe at high P-T. The results constrain the resistivity and thermal conductivity of hcp-iron to ~80(5) u Omega cm and ~100(10) W/mK, respectively, at conditions near core-mantle boundary. Our results indicate an adiabatic heat flow of ~10(1) TW through the core-mantle boundary for a liquid Fe alloy outer core, supporting a present-day geodynamo driven by thermal convection through the core's secular cooling and by compositional convection through the latent heat and gravitational energy during the inner core's solidification.",2004.12035v1 2020-08-26,"Understanding the role of Ca segregation on thermal stability, electrical resistivity and mechanical strength of nanostructured aluminum","Achieving a combination of high mechanical strength and high electrical conductivity in low-weight Al alloys requires a full understanding of the relationships between nanoscaled features and physical properties. Grain boundary strengthening through grain size reduction offers some interesting possibilities but is limited by thermal stability issues. Zener pinning by stable nanoscaled particles or grain boundary segregation are well-known strategies for stabilizing grain boundaries. In this study, the Al-Ca system has been selected to investigate the way segregation affects the combination of mechanical strength and electrical resistivity. For this purpose, an Al-Ca composite material was severely deformed by high-pressure torsion to achieve a nanoscaled structure with a mean grain size of only 25 nm. X-ray diffraction, transmission electron microscopy and atom probe tomography data revealed that the fcc Ca phase was dissolved for large levels of plastic deformation leading mainly to Ca segregations along crystalline defects. The resulting microhardness of about 300 HV is much higher than predictions based on Hall and Petch Law and is attributed to limited grain boundary mediated plasticity due to Ca segregation. The electrical resistivity is also much higher than that expected for nanostructured Al. The main contribution comes from Ca segregations that lead to a fraction of electrons reflected or trapped by grain boundaries twice larger than in pure Al. The two-phase state was investigated by in-situ and ex-situ microscopy after annealing at 200{\textdegree}C for 30 min, where precipitation of nanoscaled Al4Ca particles occurred and the mean grain size reached 35 nm. Annealing also significantly decreased electrical resistivity, but it remained much higher than that of nanostructured pure Al, due to Al/Al4Ca interfaces that reflect or trap more than 85% of electrons.",2008.11405v1 2021-02-15,"High-entropy van der Waals materials formed from mixed metal dichalcogenides, halides and phosphorus trisulfides","The charge, spin, and composition degrees of freedom in high-entropy alloy endow it with tunable valence and spin states, infinite combinations and excellent mechanical performance. Meanwhile, the stacking, interlayer, and angle degrees of freedom in van der Waals material bring it with exceptional features and technological applications. Integration of these two distinct material categories while keeping their merits would be tempting. Based on this heuristic thinking, we design and explore a new range of materials (i.e., dichalcogenides, halides and phosphorus trisulfides) with multiple metallic constitutions and intrinsic layered structure, which are coined as high-entropy van der Waals materials. Millimeter-scale single crystals with homogeneous element distribution can be efficiently acquired and easily exfoliated or intercalated in this materials category. Multifarious physical properties like superconductivity, magnetic ordering, metal-insulator transition and corrosion resistance have been exploited. Further research based on the concept of high-entropy van der Waals materials will enrich the high-throughput design of new systems with intriguing properties and practical applications.",2102.07493v2 2014-12-01,Conventional superconductivity at 190 K at high pressures,"The highest critical temperature of superconductivity Tc has been achieved in cuprates: 133 K at ambient pressure and 164 K at high pressures. As the nature of superconductivity in these materials is still not disclosed, the prospects for a higher Tc are not clear. In contrast the Bardeen-Cooper-Schrieffer (BCS) theory gives a clear guide for achieving high Tc: it should be a favorable combination of high frequency phonons, strong coupling between electrons and phonons, and high density of states. These conditions can be fulfilled for metallic hydrogen and covalent hydrogen dominant compounds. Numerous followed calculations supported this idea and predicted Tc=100-235 K for many hydrides but only moderate Tc~17 K has been observed experimentally. Here we found that sulfur hydride transforms at P~90 GPa to metal and superconductor with Tc increasing with pressure to 150 K at ~200 GPa. This is in general agreement with recent calculations of Tc~80 K for H2S. Moreover we found superconductivity with Tc~190 K in a H2S sample pressurized to P>150 GPa at T>220 K. This superconductivity likely associates with the dissociation of H2S, and formation of SHn (n>2) hydrides. We proved occurrence of superconductivity by the drop of the resistivity at least 50 times lower than the copper resistivity, the decrease of Tc with magnetic field, and the strong isotope shift of Tc in D2S which evidences a major role of phonons in the superconductivity. H2S is a substance with a moderate content of hydrogen therefore high Tc can be expected in a wide range of hydrogen-contain materials. Hydrogen atoms seem to be essential to provide the high frequency modes in the phonon spectrum and the strong electron-phonon coupling.",1412.0460v1 2021-04-12,High-speed ionic synaptic memory based on two-dimensional titanium carbide MXene,"Synaptic devices with linear high-speed switching can accelerate learning in artificial neural networks (ANNs) embodied in hardware. Conventional resistive memories however suffer from high write noise and asymmetric conductance tuning, preventing parallel programming of ANN arrays as needed to surpass conventional computing efficiency. Electrochemical random-access memories (ECRAMs), where resistive switching occurs by ion insertion into a redox-active channel address these challenges due to their linear switching and low noise. ECRAMs using two-dimensional (2D) materials and metal oxides suffer from slow ion kinetics, whereas organic ECRAMs enable high-speed operation but face significant challenges towards on-chip integration due to poor temperature stability of polymers. Here, we demonstrate ECRAMs using 2D titanium carbide (Ti3C2Tx) MXene that combines the high speed of organics and the integration compatibility of inorganic materials in a single high-performance device. Our ECRAMs combine the speed, linearity, write noise, switching energy and endurance metrics essential for parallel acceleration of ANNs, and importantly, they are stable after heat treatment needed for back-end-of-line integration with Si electronics. The high speed and performance of these ECRAMs introduces MXenes, a large family of 2D carbides and nitrides with more than 30 compositions synthesized to date, as very promising candidates for devices operating at the nexus of electrochemistry and electronics.",2104.05396v4 2022-12-06,Novel superhard structures of high-pressure C-N compounds,"Through machine learning force field accelerated structure search combined with first-principles calculations, we have studied the structures of new C-N compounds with different stoichiometric ratios, and found twelve new superhard C-N compounds, the energies of these structures are similar to c-C3N4 , which is possibly synthesized by high pressure experiment, the XRD of Pa-3(C4N) P3(C4N) and C2/m(C2N) are consistent with previous experimental data and can be used as the structural candidate. According to the macro hardness model, they are all superhard structures, with Vickers hardness over 40GPa, even, the hardness of Pa-3 (C4N) as high as 82.2GPa, and Pa-3 (C4N) combines high tensile and shear resistance. Compared with the hardness calculated by macro hardness model and bond resistance model, we obtained the relationship between the hardness and chemical concentration of C-N compounds under the two models, besides that, we also calculated the fracture toughness of these structures. According to Niu's model, P2_1/c(C4N) has the best fracture toughness, which is higher than WC in calculation, This also indicated the superior mechanical properties of the novel C-N compounds. Moreover, for nitrogen-rich structures, they have the potential to be used as high energy density, the energy density of Pa-3(CN3), P-3c1 (CN4), and I-42d (CN4) are 7.076kJ/g, 7.742kJ/g and 8.045kJ/g, which is close or higher than CL-20, therefore, the C-N compounds synthesized under high pressure have great potential as ideally superhard materials and high energy density materials(HEDMs).",2212.03009v3 2004-03-19,Influence of intermartensitic transitions on transport properties of Ni2.16Mn0.84Ga alloy,"Magnetic, transport, and x-ray diffraction measurements of ferromagnetic shape memory alloy Ni$_{2.16}$Mn$_{0.84}$Ga revealed that this alloy undergoes an intermartensitic transition upon cooling, whereas no such a transition is observed upon subsequent heating. The difference in the modulation of the martensite forming upon cooling from the high-temperature austenitic state [5-layered (5M) martensite], and the martensite forming upon the intermartensitic transition [7-layered (7M) martensite] strongly affects the magnetic and transport properties of the alloy and results in a large thermal hysteresis of the resistivity $\rho$ and magnetization $M$. The intermartensitic transition has an especially marked influence on the transport properties, as is evident from a large difference in the resistivity of the 5M and 7M martensite, $(\rho_{\mathrm{5M}} - \rho_{\mathrm{7M}})/\rho _{\mathrm{5M}} \approx 15%$, which is larger than the jump of resistivity at the martensitic transition from the cubic austenitic phase to the monoclinic 5M martensitic phase. We assume that this significant difference in $\rho$ between the martensitic phases is accounted for by nesting features of the Fermi surface. It is also suggested that the nesting hypothesis can explain the uncommon behavior of the resistivity at the martensitic transition, observed in stoichiometric and near-stoichiometric Ni-Mn-Ga alloys.",0403495v1 2004-10-10,Ultrathin epitaxial graphite: 2D electron gas properties and a route toward graphene-based nanoelectronics,"We have produced ultrathin epitaxial graphite films which show remarkable 2D electron gas (2DEG) behavior. The films, composed of typically 3 graphene sheets, were grown by thermal decomposition on the (0001) surface of 6H-SiC, and characterized by surface-science techniques. The low-temperature conductance spans a range of localization regimes according to the structural state (square resistance 1.5 kOhm to 225 kOhm at 4 K, with positive magnetoconductance). Low resistance samples show characteristics of weak-localization in two dimensions, from which we estimate elastic and inelastic mean free paths. At low field, the Hall resistance is linear up to 4.5 T, which is well-explained by n-type carriers of density 10^{12} cm^{-2} per graphene sheet. The most highly-ordered sample exhibits Shubnikov - de Haas oscillations which correspond to nonlinearities observed in the Hall resistance, indicating a potential new quantum Hall system. We show that the high-mobility films can be patterned via conventional lithographic techniques, and we demonstrate modulation of the film conductance using a top-gate electrode. These key elements suggest electronic device applications based on nano-patterned epitaxial graphene (NPEG), with the potential for large-scale integration.",0410240v1 2005-04-29,"Electromigration in thin tunnel junctions with ferromagnetic/nonmagnetic: nanoconstrictions, local heating, and direct and wind forces","Current Induced Resistance Switching (CIS) was recently observed in thin tunnel junctions with ferromagnetic (FM) electrodes \emph{i.e} FM/I/FM. This effect was attributed to electromigration of metallic atoms in nanoconstrictions in the insulating barrier (I). Here we study how the CIS effect is influenced by a thin non-magnetic (NM) Ta layer, deposited just below the AlO$_x$ insulating barrier in tunnel junctions of the type FM/NM/I/FM (FM=CoFe). Enhanced resistance switching occurs with increasing maximum applied current ($\Imax$), until a plateau of constant CIS is reached for $\Imax\sim65$ mA (CIS$\sim$60%) and above. However, such high electrical currents also lead to a large ($\sim$9%) irreversible resistance decrease, indicating barrier degradation. Anomalous voltage-current characteristics with negative derivative were also observed near $\pm\Imax$ and this effect is here attributed to heating in the tunnel junction. One observes that the current direction for which resistance switches in FM/NM/I/FM (clockwise) is opposite to that of FM/I/FM tunnel junctions (anti-clockwise). This effect will be discussed in terms of a competition between the electromigration contributions due to the so called direct and wind forces. It will be shown that the direct force is likely to dominate electromigration in the Ta (NM) layers, while the wind contribution likely dominates in the CoFe (FM) layers.",0504772v6 2007-02-05,Effect of Ir substitution in the ferromagnetic superconductor RuSr2GdCu2O8,"A detailed study of the effect caused by the partial substitution of Ru by Ir on the magnetic and superconducting properties of the ruthenocuprate Ru(1-x)Ir(x)Sr2GdCu2o8; 0 <= x <= 0.10; is presented. The combined experimental results of structural, electrical, and magnetic measurements indicate that Ir substitutes Ru for x <= 0.10 with no significant structural distortions. Ir-doping gradually suppresses both the magnetic and the superconducting states. However, all samples were observed to attain the zero-resistance state at temperatures >= 2 K up to the highest applied magnetic field of 18 T. The resistive upper-critical field Hc2 as a function of temperature has been determined for these polycrystalline samples. Values of Hc2(0) were found to be \~ 52 T, and weakly dependent on the Ir concentration. We have also observed that the superconducting transition width decreases and the slope of the resistive transition increases with increasing Ir doping, a feature which is much more pronounced at high applied magnetic fields. The double-peak structure observed in the derivative of the resistive curves has been related to an inhomogeneous nature of the physical grains which is enhanced due to the Ru substitution by Ir. This indicates that the Josephson-junction-array (JJA) model seems to be appropriated to describe the superconducting state in these ruthenocuprates. The low temperature rho(T) data along with the determined vortex thermal activation energy are consistent with a 2D vortex dynamics in these materials.",0702078v1 1997-04-04,Radiation damage to neutron and proton irradiated GaAs particle detectors,"The radiation damage in 200 um thick Schottky diodes made on semi-insulating (SI) undoped GaAs Liquid Encapsulated Czochralski (LEC) bulk material with resistivities between 0.4 and 8.9*10E7 Ohm*cm were studied using alpha-spectroscopy, signal response to minimum ionising particles (MIP), I-V and CV-measurements. The results have been analysed to investigate the influence of the substrate resistivity on the detector performance after neutron and proton irradiation. The leakage current density, signal response to alpha-particles and MIPs show a strong dependence on the resistivity before and after irradiation. An observed decrease of the electron mean free drift length before and after irradiation with increasing substrate resistivity can be explained by a model involving the different ionisation ratios of defects, which are introduced by the irradiation. Comparison of the radiation damage due to neutrons and protons gives a hardness factor of 7+-0.9 for 24 GeV/c protons. The best detectors show a response to MIPs of 5250 e- at 200 V reverse bias after a irradiation level of 2*10E14 p/cm^2.",9704002v1 2003-04-10,Students' Understanding of Direct Current Resistive Electrical Circuits,"Research has shown that both high school and university students' reasoning patterns regarding direct current resistive electric circuits often differ from the currently accepted explanations. At present, there are no standard diagnostic examinations in electric circuits. Two versions of a diagnostic instrument called Determining and Interpreting Resistive Electric circuits Concepts Tests (DIRECT) were developed, each consisting of 29 questions. The information provided by the exam provides classroom instructors a means with which to evaluate the progress and conceptual difficulties of their students and their instructional methods. It can be used to evaluate curricular packages and/or other supplemental materials for their effectiveness in overcoming students' conceptual difficulties. The analyses indicate that students, especially females, tend to hold multiple misconceptions, even after instruction. During interviews, the idea that the battery is a constant source of current was used most often in answering the questions. Students tended to focus on current in solving the problems and to confuse terms, often assigning the properties of current to voltage and/or resistance. Results indicated that students do not have a clear understanding of the underlying mechanisms of electric circuit phenomena. On the other hand, students were able to translate easily from a ""realistic"" representation of a circuit to the corresponding schematic diagram.",0304040v2 2013-05-15,"Structural ordering driven anisotropic magnetoresistance, anomalous Hall resistance and its topological overtones in full-Heusler Co2MnSi thin films","We report the evolution of crystallographic structure, magnetic ordering and electronic transport in thin films of full-Heusler alloy Co$_2$MnSi deposited on (001) MgO with annealing temperatures ($T_A$). By increasing the $T_A$ from 300$^\circ$C to 600$^\circ$C, the film goes from a disordered nanocrystalline phase to $B2$ ordered and finally to the $L2_1$ ordered alloy. The saturation magnetic moment improves with structural ordering and approaches the Slater-Pauling value of $\approx 5.0 \mu_B$ per formula unit for $T_A$ = 600$^\circ$C. At this stage the films are soft magnets with coercive and saturation fields as low as $\approx$ 7 mT and 350 mT, respectively. Remarkable effects of improved structural order are also seen in longitudinal resistivity ($\rho_{xx}$) and residual resistivity ratio. A model based upon electronic transparency of grain boundaries illucidates the transition from a state of negative $d\rho/dT$ to positive $d\rho/dT$ with improved structural order. The Hall resistivity ($\rho_{xy}$) derives contribution from the normal scattering of charge carriers in external magnetic field, the anomalous effect originating from built-in magnetization and a small but distinct topological Hall effect in the disordered phase. The carrier concentration ($n$) and mobility ($\mu$) have been extracted from the high field $\rho_{xy}$ data. The highly ordered films are characterized by $n$ and $\mu$ of 1.19$\times$ 10$^{29}$ m$^{-3}$ and 0.4 cm$^2V^{-1}s^{-1}$ at room temperature. The dependence of $\rho_{xy}$ on $\rho_{xx}$ indicates the dominance of skew scattering in our films, which shows a monotonic drop on raising the $T_A$. The topological Hall effect is analyzed for the films annealed at 300$^\circ$C. ......",1305.3453v1 2013-05-21,Observation of even denominator fractional quantum Hall effect in suspended bilayer graphene,"We investigate low-temperature magneto-transport in recently developed, high-quality multi-terminal suspended bilayer graphene devices, enabling the independent measurement of the longitudinal and transverse resistance. We observe clear signatures of the fractional quantum Hall effect, with different states that are either fully developed, and exhibit a clear plateau in the transverse resistance with a concomitant dip in longitudinal resistance, or incipient, and exhibit only a longitudinal resistance minimum. All observed states scale as a function of filling factor nu, as expected. An unprecedented even-denominator fractional state is observed at nu = -1/2 on the hole side, exhibiting a clear plateau in Rxy quantized at the expected value of 2h/e^2 with a precision of ~0.5%. Many of our observations, together with a recent electronic compressibility measurement performed in graphene bilayers on hexagonal boron-nitride (hBN) substrates, are consistent with a recent theory that accounts for the effect of the degeneracy between the N=0 and N=1 Landau levels in the fractional quantum Hall effect, and predicts the occurrence of a Moore-Read type nu = -1/2 state. Owing to the experimental flexibility of bilayer graphene --which has a gate-dependent band structure, can be easily accessed by scanning probes, and can be contacted with materials such as superconductors--, our findings offer new possibilities to explore the microscopic nature of even-denominator fractional quantum Hall effect.",1305.4761v3 2014-11-07,Resistance noise at the metal-insulator transition in thermochromic VO2 films,"Thermochromic VO2 films were prepared by reactive DC magnetron sputtering onto heated sapphire substrates and were used to make 100-nm-thick samples that were 10 {\mu}m wide and 100 micron long. The resistance of these samples changed by a factor of about 2000 in the 50 < Ts < 70 C range of temperature Ts around the ""critical"" temperature Tc between a low-temperature semiconducting phase and a high-temperature metallic-like phase of VO2. Power density spectra S(f) were extracted for resistance noise around Tc and demonstrated unambiguous 1/f behavior. Data on S(10Hz)/Rs^2 scaled as Rs^x, where Rs is sample resistance; the noise exponent x was -2.6 for Ts < Tc and +2.6 for Ts > Tc. These exponents can be reconciled with the Pennetta-Trefan-Reggiani theory [C. Pennetta, G. Trefanan, and L. Reggiani, Phys. Rev. Lett. 85, 5238 (2000)] for lattice percolation with switching disorder ensuing from random defect generation and healing in steady state. Our work hence highlights the dynamic features of the percolating semiconducting and metallic-like regions around Tc in thermochromic VO2 films.",1411.2026v1 2015-02-18,Anomalous electrical conductivity in rapidly crystallized Cu${}_{50-x}$Zr${}_{x}$ (x = 50 - 66.6) alloys,"Cu${}_{50-x}$Zr${}_{x}$ (x = 50, 54, 60 and 66.6) polycrystalline alloys were prepared by arc-melting. The crystal structure of the ingots has been examined by X-ray diffraction. Non-equilibrium martensitic phases with monoclinic structure were detected in all the alloys except Cu${}_{33.4}$Zr${}_{66.6}$. Temperature dependencies of electrical resistivity in the temperature range of T = 4 - 300 K have been measured as well as room temperature values of Hall coefficients and thermal conductivity. Electrical resistivity demonstrates anomalous behavior. At the temperatures lower than 20 K, their temperature dependencies are non-monotonous with pronounced minima. At elevated temperatures they have sufficiently non-linear character which cannot be described within framework of the standard Bloch--Gr\""{u}neisen model. We propose generalized Bloch--Gr\""{u}neisen model with variable Debye temperature which describes experimental resistivity dependencies with high accuracy. We found that both the electrical resistivity and the Hall coefficients reveal metallic-type conductivity in the Cu-Zr alloys. The estimated values of both the charge carrier mobility and the phonon contribution to thermal and electric conductivity indicate the strong lattice defects and structure disorder.",1502.05297v1 2016-05-24,Thermoelectric transport in the layered Ca$_3$Co$_{4-x}$Rh$_x$O$_9$ single crystals,"We have examined an isovalent Rh substitution effect on the transport properties of the thermoelectric oxide Ca$_3$Co$_{4}$O$_9$ using single-crystalline form. With increasing Rh content $x$, both the electrical resistivity and the Seebeck coefficient change systematically up to $x=0.6$ for Ca$_3$Co$_{4-x}$Rh$_{x}$O$_9$ samples. In the Fermi-liquid regime where the resistivity behaves as $\rho=\rho_0+AT^2$ around 120 K, the $A$ value decreases with increasing Rh content, indicating that the correlation effect is weakened by Rh $4d$ electrons with extended orbitals. We find that, in contrast to such a weak correlation effect observed in the resistivity of Rh-substituted samples, the low-temperature Seebeck coefficient is increased with increasing Rh content, which is explained with a possible enhancement of a pseudogap associated with the short-range order of spin density wave. In high-temperature range above room temperature, we show that the resistivity is largely suppressed by Rh substitution while the Seebeck coefficient becomes almost temperature-independent, leading to a significant improvement of the power factor in Rh-substituted samples. This result is also discussed in terms of the differences in the orbital size and the associated spin state between Co $3d$ and Rh $4d$ electrons.",1605.07682v1 2017-10-25,Engineering physics of superconducting hot-electron bolometer mixers,"Superconducting hot-electron bolometers are presently the best performing mixing devices for the frequency range beyond 1.2 THz, where good quality superconductor-insulator-superconductor (SIS) devices do not exist. Their physical appearance is very simple: an antenna consisting of a normal metal, sometimes a normal metal-superconductor bilayer, connected to a thin film of a narrow, short superconductor with a high resistivity in the normal state. The device is brought into an optimal operating regime by applying a dc current and a certain amount of local- oscillator power. Despite this technological simplicity its operation has been found to be controlled by many different aspects of superconductivity, all occurring simultaneously. A core ingredient is the understanding that there are two sources of resistance in a superconductor: a charge conversion resistance occurring at an normal-metal-superconductor interface and a resistance due to time- dependent changes of the superconducting phase. The latter is responsible for the actual mixing process in a non-uniform superconducting environment set up by the bias-conditions and the geometry. The present understanding indicates that further improvement needs to be found in the use of other materials with a faster energy-relaxation rate. Meanwhile several empirical parameters have become physically meaningful indicators of the devices, which will facilitate the technological developments.",1710.09136v1 2018-02-13,Multiple-Modes Scanning Probe Microscopy Characterization of Copper doped Zinc Oxide (ZnO:Cu) Thin Films,"This paper presents multiple-modes Scanning Probe Microscopy (SPM) studies on characterize resistance switching (RS), polarization rotation (PO) and surface potential changes in copper doped ZnO (ZnO:Cu) thin films. The bipolar RS behavior is confirmed by conductive Atomic Force Microscopy (c-AFM). The PO with almost 180{\deg} phase angle is confirmed by using the vertical and lateral Piezoresponse Force Microscopy (PFM). In addition, it elucidates that obvious polarization rotation behavior can be observed in the sample with increasing Cu concentration. Furthermore, correlation of the RS behavior with PO behavior has been studied by performing various mode SPM measurements on the same location. The electric field resulted from the opposite polarization orientation are corresponded to the different resistance states. It is found that the region with the polarization in downward direction has low resistance state (LRS), whereas the region with upward polarization has high resistance state (HRS). In addition, the Piezoresponse Force Spectroscopy (PFS) and Switching Spectroscopy PFM (SS-PFM) measurements further confirm that the existence of the built-in field due to the uncomplemented polarization may affect the depletion region and hence contribute to the RS behavior. In addition, Kelvin Probe Force Microscopy (KPFM) results show that, when ZnO-based thin films is subjected to negative and then followed by positive sample bias, injection charge limit current is dominated.",1802.04494v1 2019-02-11,Electrical percolation in metal wire network based strain sensors,"Metal wire networks rely on percolation paths for electrical conduction, and by suitably introducing break-make junctions on a flexible platform, a network can be made to serve as a resistive strain sensor. Several experimental designs have been proposed using networks made of silver nanowires, carbon nanotubes and metal meshes with high sensitivities. However, there is limited theoretical understanding; the reported studies have taken the numerical approach and only consider rearrangement of nanowires with strain, while the critical break-make property of the sensor observed experimentally has largely been ignored. Herein, we propose a generic geometrical based model and study distortion, including the break-make aspect, and change in electrical percolation of the network on applying strain. The result shows that when a given strain is applied, wire segments below a critical angle with respect to the applied strain direction end up breaking, leading to increased resistance of the network. The percolation shows interesting attributes; the calculated resistance increases linearly in the beginning and at a higher rate for higher strains, consistent with the experimental findings. In a real scenario, the strain direction need not necessarily be in the direction of measurement, and therefore, strain value and its direction both are incorporated into the treatment. The study reveals interesting anisotropic conduction features; strain sensitivity is higher parallel to the strain, while strain range is wider for perpendicular measurement. The percolation is also investigated on direct microscopic images of metal networks to obtain resistance-strain characteristics and identification of current percolation pathways. The findings will be important for electrical percolation in general, particularly in predicting characteristics and improvising metal network-based strain sensors.",1902.03746v1 2019-12-16,Electrical Characterization of CIGS Thin Film Solar Cells by Two and Four-Wires Probe Technique,"The characterization of thin film solar cells is of huge importance for obtaining high open circuit voltage and low recombination rates from the interfaces or within the bulk of the main materials. Among the many electrical characterization techniques, the two and four wire probe using the Cascade instrument is of interest since the resistance of the wires, and the electrical contacts can be excluded by the additional two wires in 4 wire probe configuration. In this paper, both two and four-point probes configuration are employed to characterize the CIGS chalcogenide thin film solar cells. The two wire probe has been used to measure the current-voltage characteristics of the cell which results in a huge internal resistance. Therefore, the four wire connection are also used to eliminate the lead resistance to enhance the characterization accuracy. The load resistance in the twowire probe diminishes the photogenerated current density at smaller voltage ranges. In contrast, the proposed four wire probe collects more current at higher voltages due to enhanced carrier collection efficiency from contact electrodes. The current conduction mechanism is also identified at every voltage region represented by the value of the ideality factor of that voltage region.",2002.07391v1 2020-03-31,Design and Simulation of Memristor-Based Artificial Neural Network for Bidirectional Adaptive Neural Interface,"This article proposes a general approach to the simulation and design of a multilayer perceptron (MLP) network on the basis of cross-bar arrays of metal-oxide memristive devices. The proposed approach uses the ANNM theory, tolerance theory, simulation methodology and experiment design. The tolerances analysis and synthesis process is performed for the ANNM hardware implementation on the basis of two arrays of memristive microdevices in the original 16x16 cross-bar topology being a component of bidirectional adaptive neural interface for automatic registration and stimulation of bioelectrical activity of a living neuronal culture used in robotics control system. The ANNM is trained for solving a nonlinear classification problem of stable information characteristics registered in the culture grown on a multi-electrode array. Memristive devices are fabricated on the basis of a newly engineered Au/Ta/ZrO2(Y)/Ta2O5/TiN/Ti multilayer structure, which contains self-organized interface oxide layers, nanocrystals and is specially developed to obtain robust resistive switching with low variation of parameters. An array of memristive devices is mounted into a standard metal-ceramic package and can be easily integrated into the neurointerface circuit. Memristive devices demonstrate bipolar switching of anionic type between the high-resistance state and low-resistance state and can be programmed to set the intermediate resistive states with a desired accuracy. The ANNM tuning, testing and control are implemented by the FPGA-based control subsystem. All developed models and algorithms are implemented as Python-based software.",2004.00154v1 2017-04-29,Wear-resistant thin films of MRI-230D-Mg alloy using plasma-driven electrolytic oxidation,"Wear resistant coatings were produced on a permanent mould cast MRI 230D Mg alloy by (a) PEO in silicate based electrolyte, (b) PEO in phosphate based electrolyte, (c) hybrid coatings of silicate PEO followed by laser surface alloying (LSA) with Al and Al2O3, and (d) hybrid coatings of phosphate PEO followed by LSA with Al and Al2O3. Microstructural characterization of the coatings was carried out by scanning electron microscopy (SEM) and X(ray diffraction. The tribological behavior of the coatings was investigated under dry sliding condition using linearly reciprocating ball-on-flat wear test. Both the PEO coatings exhibited a friction coefficient of about 0.8 and hybrid coatings exhibited a value of about 0.5 against the AISI 52100 steel ball as the friction partner, which were slightly reduced with the increase in applied load. The PEO coatings sustained the test without failure at 2 N load but failed at 5 N load due to micro-fracture caused by high contact stresses. The hybrid coatings did not get completely worn off at 2 N load but were completely removed exposing the substrate at 5 N load. The PEO coatings exhibited better wear resistance than the hybrid coatings and silicate PEO coatings exhibited better wear resistance than the phosphate PEO coatings. Both the PEO coatings melted/decomposed on laser irradiation and all the hybrid coatings exhibited similar microstructure and wear behavior irrespective of the nature of the primary PEO coating or laser energies. SEM examination of worn surfaces indicated abrasive wear combined with adhesive wear for all the specimens. The surface of the ball exhibited a discontinuous transfer layer after the wear test.",1705.00116v1 2018-08-01,Effect of multiband transport on charge carrier density fluctuations at the LaAlO$_3$/SrTiO$_3$ interface,"Multiband transport in superconductors is interesting both from an academic as well as an application point of view. It has been postulated that interband scattering can significantly affect the carrier dynamics in these materials. In this article we present a detailed study of the electrical transport properties of the high-mobility two-dimensional electron gas residing at the interface of LaAlO$_3$/SrTiO$_3$, a prototypical multi-band superconductor. We show, through careful measurements of the gate dependence of the magnetoresistance and resistance fluctuations at ultra-low temperatures, that transport in the superconducting regime of this system has contributions from two bands which host carriers of very different characters. We identify a gate-voltage tunable Lifshitz transition in the system and show that the resistance fluctuations have strikingly different features on either side of it. At low carrier densities, resistance noise is dominated by number-density fluctuations arising from trapping-detrapping of charge carriers from defects in the underlying SrTiO$_3$ substrate, characteristic of a single-band semiconductor. Above the Lifshitz transition, the noise presumably originates from inter-band scattering. Our work highlights the importance of inter-band scattering processes in determining the transport properties of low-dimensional systems and projects resistance fluctuation spectroscopy as a viable technique for probing the charge carrier dynamics across a Lifshitz transition.",1808.00246v1 2016-09-06,Interlayer Transport through a Graphene / Rotated-Boron-Nitride / Graphene Heterostructure,"Interlayer electron transport through a graphene / hexagonal boron-nitride (h-BN) / graphene heterostructure is strongly affected by the misorientation angle $\theta$ of the h-BN with respect to the graphene layers with different physical mechanisms governing the transport in different regimes of angle, Fermi level, and bias. The different mechanisms and their resulting signatures in resistance and current are analyzed using two different models, a tight-binding, non-equilibrium Green function model and an effective continuum model, and the qualitative features resulting from the two different models compare well. In the large-angle regime ($\theta > 4^\circ$), the change in the effective h-BN bandgap seen by an electron at the $K$ point of the graphene causes the resistance to monotonically increase with angle by several orders of magnitude reaching a maximum at $\theta = 30^\circ$. It does not affect the peak-to-valley current ratios in devices that exhibit negative differential resistance. In the small-angle regime ($\theta < 4^\circ$), Umklapp processes open up new conductance channels that manifest themselves as non-monotonic features in a plot of resistance versus Fermi level that can serve as experimental signatures of this effect. For small angles and high bias, the Umklapp processes give rise to two new current peaks on either side of the direct tunneling peak.",1609.01369v1 2018-12-13,Search for power-efficient wide-range reversible resistance modulation of $VO_2$ single crystals,"The abrupt metal insulator transition in $VO_2$ is attracting considerable interest from both fundamental and applicative angles. We report on DC I-V characteristics measured on $VO_2$ single crystals in the two-probe configuration at several ambient temperatures below the insulator-metal transition. The insulator-mixed-metal-insulator transition is induced by Joule heating above ambient temperature in the range of negative differential resistivity (NDR). In this range the stability of V(I) is governed by the load resistance $R_L$. Steady state I(V) is obtained for $R_L> |dV/dI|_{max}$ in the NDR regime. For $R_L< |dV/dI|_{max}$ there is switching between initial and final steady states associated with peaks in the Joule power, that are higher the lower $R_L$ is. The peaks caused by steep switching are superfluous and damaging the samples. On the other hand, the large $R_L$ needed for steady state is the main power consumer in the circuit at high currents. The present work is motivated by the need to avoid damaging switching in the NDR regime while reducing the power consumption in the circuit. It is shown here that large resistance modulation can be obtained under steady state conditions with reduced power consumption by increasing the ambient temperature of the device above room temperature.",1812.05702v1 2020-01-28,Pressure tuning of structural and magnetic transitions in EuAg$_4$As$_2$,"We report temperature dependent measurements of ambient pressure specific heat, magnetic susceptibility, anisotropic resistivity and thermal expansion as well as in-plane resistivity under pressure up to 20.8 kbar on single crystals of EuAg$_4$As$_2$. Based on thermal expansion and in-plane electrical transport measurements at ambient pressure this compound has two, first order, structural transitions in 80 - 120 K temperature range. Ambient pressure specific heat, magnetization and thermal expansion measurements show a cascade of up to seven transitions between 8 and 16 K associated with the ordering of the Eu$^{2+}$ moments. In-plane electrical transport is able to detect more prominent of these transitions: at 15.5, 9.9, and 8.7 K as well as a weak feature at 11.8 K at ambient pressure. Pressure dependent electrical transport data show that the magnetic transitions shift to higher temperatures under pressure, as does the upper structural transition, whereas the lower structural transition is suppressed and ultimately vanishes. A jump in resistivity, associated with the upper structural transition, decreases under pressure with an extrapolated disappearance (or a change of sign) by 30-35 kbar. In the 10 - 15 kbar range a kink in the pressure dependence of the upper structural transition temperature as well as the high and low temperature in-plane resistivities suggest that a change in the electronic structure may occur in this pressure range. The results are compared with the literature data for SrAg$_4$As$_2$.",2001.10574v1 2020-08-07,Dependable contact related parameter extraction in graphene-metal junctions,"The accurate extraction and the reliable, repeatable reduction of graphene - metal contact resistance (R$_{C}$) are still open issues in graphene technology. Here, we demonstrate the importance of following clear protocols when extracting R$_{C}$ using the transfer length method (TLM). We use the example of back-gated graphene TLM structures with nickel contacts, a complementary metal oxide semiconductor compatible metal. The accurate extraction of R$_{C}$ is significantly affected by generally observable Dirac voltage shifts with increasing channel lengths in ambient conditions. R$_{C}$ is generally a function of the carrier density in graphene. Hence, the position of the Fermi level and the gate voltage impact the extraction of R$_{C}$. Measurements in high vacuum, on the other hand, result in dependable extraction of R$_{C}$ as a function of gate voltage owing to minimal spread in Dirac voltages. We further assess the accurate measurement and extraction of important parameters like contact-end resistance, transfer length, sheet resistance of graphene under the metal contact and specific contact resistivity as a function of the back-gate voltage. The presented methodology has also been applied to devices with gold and copper contacts, with similar conclusions.",2008.03218v1 2021-05-18,"On the role of boron, carbon and zirconium on hot cracking and creep resistance of additively manufactured polycrystalline superalloys","We investigate the hot cracking susceptibility and creep resistance of three versions of a nickel-based superalloy with different contents of boron, carbon and zirconium fabricated by laser powder bed fusion. Crack-free and creep resistant components are achieved for alloys with boron, carbon and no zirconium. We then rationalize this result by evaluating how boron, carbon and zirconium are distributed at grain boundaries in the as-built and heat-treated microstructures of an alloy containing all these elements. Observations are conducted by scanning and transmission electron microscopy, and atom probe tomography. In the as-built microstructure, boron, carbon and zirconium segregate at high-angle grain boundaries as a result of solute partitioning to the liquid and limited solid-state diffusion during solidification and cooling. After heat-treatment, the amount of boron and carbon segregating at grain boundaries increases significantly. In contrast, zirconium is not found at grain boundaries but it partitions at the gamma' precipitates formed during the heat treatment. The presence of zirconium at grain boundaries in the as-built condition is known to be susceptible to enhance hot cracking, while its absence in the heat-treated microstructure strongly suggests that this element has no major effect on the creep resistance. Based on our observations, we propose alloy design guidelines to at the same time avoid hot cracking during fabrication and achieve the required creep performance after heat-treatment.",2105.08307v1 2021-07-13,"Reactivity of the Si(100)-2$\times$1-Cl surface with respect to PH$_3$, PCl$_3$, and BCl$_3$: Comparison with PH$_3$ on Si(100)-2$\times$1-H","Despite the interest in a chlorine monolayer on Si(100) as an alternative to hydrogen resist for atomic-precision doping, little is known about its interaction with dopant-containing molecules. We used the density functional theory to evaluate whether a chlorine monolayer on Si(100) is suitable as a resist for \ce{PH3}, \ce{PCl3}, and \ce{BCl3} molecules. We calculated reaction pathways for \ce{PH3}, \ce{PCl3}, and \ce{BCl3} adsorption on a bare and Cl-terminated Si(100)-2$\times$1 surface, as well as for \ce{PH3} adsorption on H-terminated Si(100)-2$\times$1, which is widely used in current technologies for atomically precise doping of Si(100) with phosphorus. It was found that the Si(100)-2$\times$1-Cl surface has a higher reactivity towards phosphine than Si(100)-2$\times$1-H, and, therefore, unpatterned areas are less protected from undesirable incorporation of \ce{PH3} fragments. On the contrary, the resistance of the Si(100)-2$\times$1-Cl surface against the chlorine-containing molecules turned out to be very high. Several factors influencing reactivity are discussed. The results reveal that phosphorus and boron trichlorides are well-suited for doping a patterned Cl-resist by donors and acceptors, respectively.",2107.06168v1 2022-10-18,In-plane electronic anisotropy revealed by interlayer resistivity measurements on the iron-based superconductor parent compound CaFeAsF,"Both cuprates and iron-based superconductors demonstrate nematicity, defined as the spontaneous breaking of rotational symmetry in electron systems. The nematic state can play a role in the high-transition-temperature superconductivity of these compounds. However, the microscopic mechanism responsible for the transport anisotropy in iron-based compounds remains debatable. Here, we investigate the electronic anisotropy of CaFeAsF by measuring its interlayer resistivity under magnetic fields with varying field directions. Counterintuitively, the interlayer resistivity was larger in the longitudinal configuration ($B \parallel I \parallel c$) than in the transverse one ($B \perp I \parallel c$). The interlayer resistivity exhibited a so-called coherence peak under in-plane fields and was highly anisotropic with respect to the in-plane field direction. At $T$ = 4 K and $B$ = 14 T, the magnetoresistance $\Delta\rho/\rho_0$ was seven times larger in the $B \parallel b_o$ than in the $B \parallel a_o$ configuration. Our theoretical calculations of the conductivity based on the first-principles electronic band structure qualitatively reproduced the above observations but underestimated the magnitudes of the observed features. The proposed methodology can be a powerful tool for probing the nematic electronic state in various materials.",2210.09533v2 2023-11-15,Transport properties of strongly correlated Fermi systems,"In our short review, we consider the transport properties of strongly correlated Fermi systems like heavy fermion metals and high-$T_c$ superconductors. Their transport properties are defined by strong inter-particle interaction forming flat bands in these compounds. Indeed, in contrast to the behavior of the transport properties of conventional metals, the strongly correlated compounds exhibit the linear in temperature resistivity, $\rho(T)\propto T$. We analyze the magnetoresistance and show that it under the application of magnetic field becomes negative. It is shown that near a quantum phase transition, when the density of electronic states diverges, semiclassical physics remains applicable to describe the resistivity $\rho$ of strongly correlated metals due to the presence of a transverse zero-sound collective mode, representing the phonon mode in solids. We demonstrate that when $T$ exceeds the extremely low Debye temperature $T_D$, the resistivity $\rho(T)$ changes linearly with $T$, since the mechanism of formation of the $T$-dependence $\rho(T)$ is similar electron-phonon mechanism, which predominates at high temperatures in ordinary metals. Thus, in the region of $T$-linear resistance, electron-phonon scattering leads to a lifetime of $\tau$ quasiparticles practically independent of the material, which is expressed as the ratio of the Planck constant $\hbar$ to the Boltzmann constant constant $k_B$, $T\tau\sim \hbar/k_B$. We explain that due to the non-Fermi-liquid behavior the real part of the frequency-dependent optical conductivity $\sigma^R_{opt}(\omega)$ exhibits a scaling behavior, and demonstrates the unusual power law behavior $\sigma^R_{opt}(\omega)\propto\omega^{-1}$, rather than the well-known one shown by conventional metals, $\sigma^R_{opt}(\omega)\propto\omega^{-2}$.",2311.08974v1 2024-01-26,First-principles methodology for studying magnetotransport in narrow-gap semiconductors: an application to Zirconium Pentatelluride ZrTe5,"The origin of anomalous resistivity peak and accompanied sign reversal of Hall resistivity of ZrTe$_5$ has been under debate for a long time. Although various theoretical models have been proposed to account for these intriguing transport properties, a systematic study from first principles view is still lacking. In this work, we present a first principles calculation combined with Boltzmann transport theory to investigate the transport properties in narrow-gap semiconductors at different temperatures and doping densities within the relaxation time approximation. Regarding the sensitive temperature-dependent chemical potential and relaxation time of semiconductors, we take proper approximation to simulate these two variables, and then comprehensively study the transport properties of ZrTe$_5$ both in the absence and presence of an applied magnetic field. Without introducing topological phases and correlation interactions, we qualitatively reproduced crucial features observed in experiments, including zero-field resistivity anomaly, nonlinear Hall resistivity with sign reversal, and non-saturating magnetoresistance at high temperatures. Our calculation allows a systematic interpretation of the observed properties in terms of multi-carrier and Fermi surface geometry. Our method can be extended to other narrow-gap semiconductors and further pave the way to explore interesting and novel transport properties of this field.",2401.15151v1 2016-12-09,Characterization of Fully Depleted CMOS Active Pixel Sensors on High Resistivity Substrates for Use in a High Radiation Environment,"Depleted CMOS active sensors (DMAPS) are being developed for high-energy particle physics experiments in high radiation environments, such as in the ATLAS High Luminosity Large Hadron Collider (HL-LHC). Since charge collection by drift is mandatory for harsh radiation environment, the application of high bias voltage to high resistive sensor material is needed. In this work, a prototype of a DMAPS was fabricated in a 150nm CMOS process on a substrate with a resistivity of >2 k{\Omega}cm that was thinned to 100 {\mu}m. Full depletion occurs around 20V, which is far below the breakdown voltage of 110 V. A readout chip has been attached for fast triggered readout. Presented prototype also uses a concept of sub-pixel en/decoding three pixels of the prototype chip are readout by one pixel of the readout chip. Since radiation tolerance is one of the largest concerns in DMAPS, the CCPD_LF chip has been irradiated with X-rays and neutrons up to a total ionization dose of 50 Mrad and a fluence of 10E15neq/cm2, respectively.",1612.03154v1 2022-03-14,Photomultipliers as High Rate Radiation-Resistant In-Situ Sensors in Future Experiments,"In the Energy Frontier we suggest developing high rate (100 MHz) finely segmented forward calorimetry preradiators with time resolution <50 ps which will survive the first 1-2 Lint of incident high radiation doses, protecting forward calorimeters 3 0, is the strongest in materials with the largest normal-state anisotropy, regardless of whether anisotropy is varied by changing the carrier concentration or by comparing a variety of optimally-doped compounds.",9908190v1 2009-04-10,Transition of stoichiometricSr2VO3FeAs to a superconducting state at 37.2 K,"The superconductor Sr4V2O6Fe2As2 with transition temperature at 37.2 K has been fabricated. It has a layered structure with the space group of p4/nmm, and with the lattice constants a = 3.9296Aand c = 15.6732A. The observed large diamagnetization signal and zero-resistance demonstrated the bulk superconductivity. The broadening of resistive transition was measured under different magnetic fields leading to the discovery of a rather high upper critical field. The results also suggest a large vortex liquid region which reflects high anisotropy of the system. The Hall effect measurements revealed dominantly electron-like charge carriers in this material. The superconductivity in the present system may be induced by oxygen deficiency or the multiple valence states of vanadium.",0904.1732v5 2014-12-25,Carbon Nanotube Based Delay Model For High Speed Energy Efficient on Chip Data Transmission Using: Current Mode Technique,"Speed is a major concern for high density VLSI networks. In this paper the closed form delay model for current mode signalling in VLSI interconnects has been proposed with resistive load termination. RLC interconnect line is modelled using characteristic impedance of transmission line and inductive effect. The inductive effect is dominant at lower technology node is modelled into an equivalent resistance. In this model first order transfer function is designed using finite difference equation, and by applying the boundary conditions at the source and load termination. It has been observed that the dominant pole determines system response and delay in the proposed model. Using CNIA tool (carbon nanotube interconnect analyzer) the interconnect line parameters has been estimated at 45nm technology node. The novel proposed current mode model superiority has been validated for CNT type of material. It superiority factor remains to 66.66% as compared to voltage mode signalling. And current mode dissipates 0.015pJ energy where as VM consume 0.045pJ for a single bit transmission across the interconnect over CNT material. Secondly the damping factor of a lumped RLC circuit is shown to be a useful figure of merit.",1412.7818v1 2015-03-29,Edge-channel interferometer at the graphene quantum Hall pn junction,"We demonstrate a quantum Hall edge-channel interferometer in a high-quality graphene pn junction under a high magnetic field. The co-propagating p and n quantum Hall edge channels traveling along the pn interface functions as a built-in Aharanov-Bohm-type interferometer, the interferences in which are sensitive to both the external magnetic field and the carrier concentration. The trajectories of peak and dip in the observed resistance oscillation are well reproduced by our numerical calculation that assumes magnetic flux quantization in the area enclosed by the co-propagating edge channels. Coherent nature of the co-propagating edge channels are confirmed by the checkerboard-like pattern in the dc-bias and magnetic-field dependences of the resistance oscillations.",1503.08385v1 2017-11-16,Anisotropic magnetic properties of the ferromagnetic semiconductor CrSbSe$_3$,"Single crystals of CrSbSe$_3$, a structurally pseudo-one-dimensional ferromagnetic semiconductor, were grown using a high-temperature solution growth technique and were characterized by x-ray diffraction, anisotropic, temperature- and field-dependent magnetization, temperature-dependent resistivity and optical absorption measurements. A band gap of 0.7 eV was determined from both resistivity and optical measurements. At high temperatures, CrSbSe$_3$ is paramagnetic and isotropic with a Curie-Weiss temperature of $\sim$145 K and an effective moment of $\sim$4.1 $\mu_B$/Cr. A ferromagnetic transition occurs at $T_c$ = 71 K. The $a$-axis, perpendicular to the chains in the structure, is the magnetic easy axis, while the chain axis direction, along $b$, is the hard axis. Magnetic isotherms measured around $T_c$ do not follow the behavior predicted by simple mean field critical exponents for a second order phase transition. A tentative set of critical exponents is estimated based on a modified Arrott plot analysis, giving $\beta\sim$0.25, $\gamma\sim$1.38 and $\delta\sim$6.6.",1711.06342v1 2018-05-18,Search for alternative magnetic tunnel junctions based on all-Heusler stacks,"By imposing the constraints of structural compatibility, stability and a large tunneling magneto-resistance, we have identified the Fe$_3$Al/BiF$_3$/Fe$_3$Al stack as a possible alternative to the well-established FeCoB/MgO/FeCoB in the search for a novel materials platform for high-performance magnetic tunnel junctions. Various geometries of the Fe$_3$Al/BiF$_3$/Fe$_3$Al structure have been analyzed, demonstrating that a barrier of less than 2~nm yields a tunneling magneto-resistance in excess of 25,000~\% at low bias, without the need for the electrodes to be half-metallic. Importantly, the presence of a significant spin gap in Fe$_3$Al for states with $\Delta_1$ symmetry along the stack direction makes the TMR very resilient to high voltages.",1805.08603v1 2019-09-23,High Throughput Production of Transparent Conductive Single-Walled Carbon Nanotube Films via Advanced Floating Catalyst Chemical Vapor Deposition,"Single-walled carbon nanotube (SWCNT) films are promising materials for transparent conductive films (TCFs) with potential applications in flexible displays, touch screens, solar cells and solid-state lighting1,2. However, further reductions in resistivity and in cost of SWCNT films are necessary for high quality TCF products3. Here, we report an improved floating catalyst chemical vapor deposition method to directly and continuously produce ultrathin and freestanding SWCNT films at the hundred meter-scale. Both carbon conversion efficiency and SWCNT TCF yield are increased by three orders of magnitude relative to the conventional floating catalyst chemical vapor deposition. After doping, the film manifests a sheet resistance of 40 ohm/sq. at 90% transmittance, representing record performance for large-scale SWCNT films. Our work provides a new avenue to accelerate the industrialization of SWCNT films as TCFs.",1909.10189v1 2020-03-24,XUV Induced Bleaching of a Tin Oxo Cage Photoresist Studied by High Harmonic Absorption Spectroscopy,"Inorganic molecular materials such as tin oxo cages are a promising generation of photoresists compatible with the demands of the recently developed Extreme UltraViolet (EUV) lithography technology. Therefore, a detailed understanding of the photon-induced reactions which occur in photoresists after exposure is important. We used XUV broadband laser pulses in the range of 25-40 eV from a table-top high-harmonic source to expose thin films of the tin oxo cage resist to shed light on some of the photo-induced chemistry via XUV absorption spectroscopy. During the exposure, the transmitted spectra were recorded and a noticeable absorbance decrease was observed in the resist. Dill parameters were extracted to quantify the XUV induced conversion and compared to EUV exposure results at 92 eV. Based on the absorption changes, we estimate that approximately 60% of tin-carbon bonds are cleaved at the end of the exposure.",2003.10961v1 2017-03-18,Discovering the Building Blocks of Atomic Systems using Machine Learning,"Machine learning has proven to be a valuable tool to approximate functions in high-dimensional spaces. Unfortunately, analysis of these models to extract the relevant physics is never as easy as applying machine learning to a large dataset in the first place. Here we present a description of atomic systems that generates machine learning representations with a direct path to physical interpretation. As an example, we demonstrate its usefulness as a universal descriptor of grain boundary systems. Grain boundaries in crystalline materials are a quintessential example of a complex, high-dimensional system with broad impact on many physical properties including strength, ductility, corrosion resistance, crack resistance, and conductivity. In addition to modeling such properties, the method also provides insight into the physical ""building blocks"" that influence them. This opens the way to discover the underlying physics behind behaviors by understanding which building blocks map to particular properties. Once the structures are understood, they can then be optimized for desirable behaviors.",1703.06236v1 2019-06-06,Modeling the effect of microstructure on elastic wave propagation in platelet-reinforced composites and ceramics,"Dense ceramics are irreplaceable in applications requiring high mechanical stiffness, chemical and temperature resistance and low weight. To improve their toughness, ceramics can be reinforced with elongated inclusions. Recent manufacturing strategies have been developed to control the orientations of disc-like micro-particles in polymeric and ceramic matrices and to build periodic microstructures. Given the infinite number of possible microstructures available, modeling tools are required to select the potentially best design. Periodic microstructures can be involved in elastic wave scattering to dissipate mechanical energy from vibrations. In this paper, a model is proposed to determine the frequency bandgaps associated to periodic architectures in composites and ceramics and the influence of microstructural parameters are investigated. The results are used to define guidelines for the future fabrication of hard bulk ceramic materials that combine traditional ceramic properties with high vibration resistance.",1906.02582v1 2020-08-28,Tunnel magnetoresistance in scandium nitride magnetic tunnel junctions using first principles,"The magnetic tunnel junction is a cornerstone of spintronic devices and circuits, providing the main way to convert between magnetic and electrical information. In state-of-the-art magnetic tunnel junctions, magnesium oxide is used as the tunnel barrier between magnetic electrodes, providing a uniquely large tunnel magnetoresistance at room temperature. However, the wide bandgap and band alignment of magnesium oxide-iron systems increases the resistance-area product and causes challenges of device-to-device variability and tunnel barrier degradation under high current. Here, we study using first principles narrower-bandgap scandium nitride tunneling properties and transport in magnetic tunnel junctions in comparison to magnesium oxide. These simulations demonstrate a high tunnel magnetoresistance in Fe/ScN/Fe MTJs via {\Delta}_1 and {\Delta}_2' symmetry filtering with low wavefunction decay rates, allowing a low resistance-area product. The results show that scandium nitride could be a new tunnel barrier material for magnetic tunnel junction devices to overcome variability and current-injection challenges.",2008.12770v1 2020-11-07,Thickness-dependent quantum transport of Weyl fermions in ultra-high-quality SrRuO3 films,"The recent observation of Weyl fermions in the itinerant 4d ferromagnetic perovskite SrRuO3 points to this material being a good platform for exploring novel physics related to a pair of Weyl nodes in epitaxial heterostructures. In this letter, we report the thickness-dependent magnetotransport properties of ultra-high-quality epitaxial SrRuO3 films grown under optimized conditions on SrTiO3 substrates. Signatures of Weyl fermion transport, i.e., unsaturated linear positive magnetoresistance accompanied by a quantum oscillation having a {\pi} Berry phase, were observed in films with thicknesses as small as 10 nm. Residual resistivity increased with decreasing film thickness, indicating disorder near the interface between SrRuO3 and the SrTiO3 substrate. Since this disorder affects the magnetic and electrical properties of the films, the Curie temperature decreases and the coercive field increases with decreasing thickness. Thickness-dependent magnetotransport measurements revealed that the threshold residual resistivity ratio (RRR) to observe Weyl fermion transport is 21. These results provide guidelines for realizing quantum transport of Weyl fermions in SrRuO3 near heterointerfaces.",2011.03670v1 2021-05-11,Exploring the Correlation between Solvent Diffusion and Creep Resistance of Mg-Ga HCP Alloys from High Throughput Liquid-Solid Diffusion Couple,"The liquid-solid diffusion couple technique, supported by phenomenological analysis and nano-indentation tests, is proposed on account of the relatively low melting points of Mg to explore the diffusion mobility and creep deformation. The potential of this strategy is demonstrated in Mg-Ga hcp alloys where Ga solute (i.e. impurity) and Mg solvent diffusions in hcp Mg-Ga alloys were both unveiled. It was followed by mapping the compressive creep behavior via nanoindentation along the composition arrays within the same Mg-Ga couple sample. The compressive creep resistance of Mg-Ga hcp alloys increased with the Ga content, and this enhancement was similar to the one found in Mg-Zn alloys and superior to the one reported in Mg-Al alloys though Al is a slower impurity diffuser in hcp-Mg than Zn and Ga. Thereby, the solvent diffusion and its variation with the composition, rather than the solute diffusion, was suggested to govern the creep properties at high temperatures and low stresses.",2105.05096v1 2021-08-30,Out-of-Plane Resistance Switching of 2D Bi2O2Se at Nanoscale,"2D bismuth oxyselenide (Bi2O2Se) with high electron mobility shows great potential for nanoelectronics. Although in-plane properties of Bi2O2Se have been widely studied, its out-ofplane electrical transport behavior remains elusive, despite its importance in fabricating devices with new functionality and high integration density. Here, we study the out-of-plane electrical properties of 2D Bi2O2Se at nanoscale by conductive atomic force microscope. We find that hillocks with tunable heights and sizes are formed on Bi2O2Se after applying vertical electrical field. Intriguingly, such hillocks are conductive in vertical direction, resulting in a previously unknown out-of-plane resistance switching in thick Bi2O2Se flakes while ohmic conductive characteristic in thin ones. Furthermore, we observe the transformation from bipolar to stable unipolar conduction in thick Bi2O2Se flake possessing such hillocks, suggesting its potential to function as a selector in vertical devices. Our work reveals unique out-of-plane transport behavior of 2D Bi2O2Se, providing the basis for fabricating vertical devices based on this emerging 2D material.",2108.13240v1 2004-07-07,Properties of MgB2 thin films with carbon doping,"We have studied structural and superconducting properties of MgB2 thin films doped with carbon during the hybrid physical-chemical vapor deposition process. A carbon-containing metalorganic precursor bis(cyclopentadienyl)magnesium was added to the carrier gas to achieve carbon doping. As the amount of carbon in the films increases, the resistivity increases, Tc decreases, and the upper critical field increases dramatically as compared to the clean films. The self-field Jc in the carbon-doped films is lower than that in the clean films, but Jc remains relatively high to much higher magnetic fields, indicating stronger pinning. Structurally, the doped films are textured with nano-grains and highly resistive amorphous areas at the grain boundaries. The carbon doping approach can be used to produce MgB2 materials for high magnetic field applications.",0407146v1 2006-01-30,Growth of high quality large area MgB2 thin films by reactive evaporation,"We report a new in-situ reactive deposition thin film growth technique for the production of MgB2 thin films which offers several advantages over all existing methods and is the first deposition method to enable the production of high-quality MgB2 films for real-world applications. We have used this growth method, which incorporates a rotating pocket heater, to deposit MgB2 films on a variety of substrates, including single-crystalline, polycrystalline, metallic, and semiconductor materials up to 4"" in diameter. This technique allows growth of double-sided, large-area films in the intermediate temperature range of 400 to 600 degrees C. These films are clean, well-connected, and consistently display Tc values of 38 to 39 K with low resistivity and residual resistivity values. They are also robust and uncommonly stable upon exposure to atmosphere and water.",0601669v1 2017-03-27,"Machining of Spherical Component Fabricated by Selected Laser Melting, Part II: Application of Ti in Biomedical","Ti and Ti-Based alloys have unique properties such as high strength, low density and excellent corrosion resistance. These properties are essential for the manufacture of lightweight and high strength components for biomedical applications. In this paper, Ti properties such as metallurgy, mechanical properties, surface modification, corrosion resistance, biocompatibility and osseointegration in biomedical applications have been discussed. This paper also analyses the advantages and disadvantages of various Ti manufacturing processes for biomedical applications such as casting, powder metallurgy, cold and hot working, machining, laser engineering net shaping, superplastic forming, forging and ring rolling. The contributions of this research are twofold, firstly scrutinizing the behaviour of Ti and Ti-Based alloys in-vivo and in-vitro experiments in biomedical applications to determine the factors leading to failure, and secondly strategies to achieve desired properties essential to improving the quality of patient outcomes after receiving surgical implants. Future research will be directed toward manufacturing of Ti for medical applications by improving the production process, for example using optimal design approaches in additive manufacturing and investigating alloys containing other materials in order to obtain better medical and mechanical characteristics.",1703.10045v1 2021-10-28,Analysis of Prospective Elements and Crystal Lattice Structures via Computer Algorithms to Identify Standard Temperature Pressure (STP) Superconductors,"Superconductors have the potential to revolutionize technology due to their ability to have zero electrical resistance. However, superconductor materials require either low temperatures or high pressures to function in a superconductive state. Thus, researchers are now on the search for the first-ever room temperature, ambient pressure superconductor. Yet, recent discoveries have only shown superconductors that work at low temperatures with ambient pressure or room temperature with high pressures. The region between these two extremes has not been identified due to the number of variables that affect superconductivity. To reduce the number of permutations that need to be tested to identify the first STP superconductor I propose the use of a computer algorithm designed to test various crystal structures of superconducting materials and combinations of elements that will have zero electrical resistance and exhibit the Meisner effect. Some elemental superconductors that have the highest critical temperature at standard pressure are V, Zr, La, Hf, Re, Th, Pa, U, and Am. The elements once combined with other elements in the right crystalline structure can produce a metastable state where the superconductors will keep their physical characteristics once they form.",2110.15201v1 2022-07-28,Pressure induced 3D strain in 2D Graphene,"Two-dimensional (2D) materials such as graphene offer a variety of outstanding properties for a wide range of applications. Their transport properties in particular present a rich field of study. However, the studies of transport properties of graphene under pressure are mostly limited to $\sim$1 GPa, largely due to the technical challenges and difficulties of placing graphene inside a diamond anvil cell (DAC) and maintaining good electrical contacts under pressure. We developed a novel technique allowing for direct measurements of the transport properties of high quality chemical vapor deposition (CVD) monolayer graphene under pressures. Combined Raman spectroscopic and direct resistivity measurements on pure monolayer graphene up to 40 GPa shows an effective out of plane stiffness of $c_{33}$=0.26$\pm_{.09}^{.11}$ GPa, and observe relatively constant resistances with pressure, suggesting high pressure as a useful technique for producing large biaxial strains within graphene.",2207.14183v1 2023-07-12,The Collaborative Effects of Intrinsic and Extrinsic Impurities in Low RRR SRF Cavities,"The superconducting radio-frequency (SRF) community has shown that introducing certain impurities into high-purity niobium can improve quality factors and accelerating gradients. We question why some impurities improve RF performance while others hinder it. The purpose of this study is to characterize the impurity profile of niobium with a low residual resistance ratio (RRR) and correlate these impurities with the RF performance of low RRR cavities so that the mechanism of impurity-based improvements can be better understood and improved upon. The combination of RF testing and material analysis reveals a microscopic picture of why low RRR cavities experience low temperature-dependent BCS resistance behavior more prominently than their high RRR counterparts. We performed surface treatments, low temperature baking and nitrogen-doping, on low RRR cavities to evaluate how the intentional addition of oxygen and nitrogen to the RF layer further improves performance through changes in the mean free path and impurity profile. The results of this study have the potential to unlock a new understanding on SRF materials and enable the next generation of SRF surface treatments.",2307.06259v1 2023-02-15,An experimental high-throughput to high-fidelity study towards discovering Al-Cr containing corrosion-resistant compositionally complex alloys,"Compositionally complex alloys hold the promise of simultaneously attaining superior combinations of properties, such as corrosion resistance, light-weighting, and strength. Achieving this goal is a challenge due in part to a large number of possible compositions and structures in the vast alloy design space. High-throughput methods offer a path forward, but a strong connection between the synthesis of an alloy of a given composition and structure with its properties has not been fully realized to date. Here, we present the rapid identification of corrosion-resistant alloys based on combinations of Al and Cr in a base Al-Co-Cr-Fe-Ni alloy. Previously unstudied alloy stoichiometries were identified using a combination of high-throughput experimental screening coupled with key metallurgical and electrochemical corrosion tests, identifying alloys with excellent passivation behavior. The alloy native oxide performance and its self-healing attributes were probed using rapid tests in deaerated 0.1 mol/L H2SO4. Importantly, a correlation was found between the electrochemical impedance modulus of the exposure-modified air-formed film and self-healing rate of the CCAs. Multi-element extended x-ray absorption fine structure analyses connected more ordered type chemical short-range order in the Ni-Al 1st nearest-neighbor shell to poorer corrosion resistance. This report underscores the utility of high throughput exploration of compositionally complex alloys for the identification and rapid screening of a vast stoichiometric space.",2302.07988v2 2021-04-06,"In-situ dispersion of electrospun nanofibers in PDMS for fabrication of high strength, transparent nanocomposites","The polymer nanocomposites find applications in diverse areas ranging from smart materials to bioengineering. They are developed by dispersion of nanomaterials in a bulk phase of a polymeric material. Although several methods facilitate efficient dispersion of nanomaterials in a bulk polymer matrix to create nanocomposites, majority of them follows heat, beat and treat processes. These processes are high energy demanding processes. Moreover, the challenge increases when nanomaterials need to be dispersed in a viscous polymeric material. This results in spatial heterogeneity in the dispersion of nanomaterials, eventually leading to compromised mechanical properties of a nanocomposite. Therefore, in the current work, we propose an in-situ, on-step fabrication process of polydimethylsiloxane (PDMS) nanocomposites. Electrospun polyvinyl alcohol (PVA) nanofibers are homogenously dispersed in a PDMS matrix to create a high strength, transparent PDMS nanocomposite. The homogenous dispersion of nanofibers in PDMS matrix is characterised by scanning electron microscopy (SEM), confocal imaging and rheological studies. Further, the prepared PDMS nanocomposite exhibits improved mechanical strength and comparable optical transparency in comparison to native PDMS. Hence, the fabricated PDMS nanocomposites, being resistant to mechanical stress and optically transparent, will find applications as transdermal patches, flexible electronics, microfluidic devices and others.",2104.02418v1 2022-04-12,Bayesian optimization with experimental failure for high-throughput materials growth,"A crucial problem in achieving innovative high-throughput materials growth with machine learning and automation techniques, such as Bayesian optimization (BO) and robotic experimentation, has been a lack of an appropriate way to handle missing data due to experimental failures. Here, we propose a new BO algorithm that complements the missing data in the optimization of materials growth parameters. The proposed method provides a flexible optimization algorithm capable of searching a wide multi-dimensional parameter space. We demonstrate the effectiveness of the method with simulated data as well as in its implementation for actual materials growth, namely machine-learning-assisted molecular beam epitaxy (ML-MBE) of SrRuO3, which is widely used as a metallic electrode in oxide electronics. Through the exploitation and exploration in a wide three-dimensional parameter space, while complementing the missing data, we attained tensile-strained SrRuO3 film with a high residual resistivity ratio of 80.1, the highest among tensile-strained SrRuO3 films ever reported, in only 35 MBE growth runs.",2204.05452v1 2023-08-30,Target tests for the ILC positron source Talk presented at the International Workshop on Future Linear Colliders (LCWS2023),"The positron source is an essential component of the International Linear Collider (ILC) and is an area that poses some design challenges. One consideration is the material for the target, where the 1014 positrons per second for the ILC are generated. The potential material would need to be able to resist the high load created by the intense high energy photon beam. One of such candidates is the titanium alloy Ti-6Al-4V, for which the results of material tests with 3.5 MeV electrons are shown. The material was characterized after the irradiation by high-energy X-ray diffraction (HE-XRD) and changes caused by the irradiation to the crystal structure were studied. These tests revealed there was only minimal change in the phase fractions and crystal structure of the material under conditions as expected for the ILC.",2308.15916v1 2019-08-16,Ab initio phonon transport across grain boundaries in graphene using machine learning based on small dataset,"Establishing the structure-property relationship for grain boundaries (GBs) is critical for developing next generation functional materials, but has been severely hampered due to its extremely large configurational space. Atomistic simulations with low computational cost and high predictive power are strongly desirable, but the conventional simulations using empirical interatomic potentials and density functional theory suffer from the lack of predictive power and high computational cost, respectively. A machine learning interatomic potential (MLIP) recently emerged but often requires an extensive size of the training dataset, making it a less feasible approach. Here we demonstrate that an MLIP trained with a rationally designed small training dataset can predict thermal transport across GBs in graphene with ab initio accuracy at an affordable computational cost. In particular, we employed a rational approach based on the structural unit model to find a small set of GBs that can represent the entire configurational space and thus can serve as a cost-effective training dataset for the MLIP. Only 5 GBs were found to be enough to represent the entire configurational space of graphene GBs. Using the atomistic Green's function approach and the MLIP, we revealed that the structure-thermal resistance relation in graphene does not follow the common understanding that large dislocation density causes larger thermal resistance. In fact, thermal resistance is nearly independent of dislocation density at room temperature and is higher when the dislocation density is small at sub-room temperature. We explain this intriguing behavior with the buckling near a GB causing a strong scattering of flexural phonon modes.",1909.02386v3 2022-02-18,Synergism between B and Nb improves fire resistance in microalloyed steels,"The development of new fire-resistant steels represents a challenge in materials science and engineering of utmost importance. Alloying elements such as Nb and Mo are generally used to improve the strength at both room- and high-temperatures due to, for example, the formation of precipitates and harder microconstituents. In this study we show alternatively that the addition of small amounts of boron in Nb-microalloyed steels may play a crucial role in maintaining the mechanical properties at high temperatures. The 66\,\% yield-strength criteria for fire resistance is achieved at $\approx 574$\,{\deg}C for a boron steel, whereas without boron this value reaches $\approx 460$\,{\deg}C, a remarkable boron-induced mechanical strengthening enhancement. DFT calculations show that boron additions can lower the vacancy formation energy when compared to pure ferrite and, for Nb-B steels, there is a further 24\,\% reduction, suggesting that the boron-niobium combination acts as an effective pinning-based strengthening agent.",2202.09197v1 2020-07-28,Good Practice Guide on the electrical characterization of graphene using non-contact and high-throughput methods,"The electrical characterisation of graphene, either in plane sheets or in properly geometrised form can be approached using non-contact methods already employed for thin film materials. The extraordinary thinness (and, correspondingly, the volume) of graphene, however, makes the proper application of these methods difficult. The electrical properties of interest (sheet electrical resistivity/conductivity, concentration and mobility of charge carriers) must be indirectly derived from the measurement outcome by geometrical and electrical modelling; the assumptions behind such models (e.g., uniformity and isotropy, effective value of the applied fields, etc.) require careful consideration. The traceability of the measurement to the International System of units and a proper expression of measurement uncertainty is an issue. This guide focuses on non-contact and high-throughput methods, that are methods where the graphene sample surface is not physically contacted with any metallic electrodes at any stage. A companion guide about contact methods is also available. The methods discussed are: - Measurement of surface potential and work function using Scanning Kelvin Probe Microscopy (SKPM); - Measurement of sheet resistance by Microwave Resonant Cavity; - Measurement of sheet resistance by Terahertz time-domain spectroscopy (THz-TDS); For each method, a corresponding measurement protocol is discussed, which describes: - The measurement principle; - Sample requirements and preparation; - A description of the measurement equipment / apparatus; - Calibration standards and ways to achieve a traceable measurement;",2007.14047v1 2020-12-08,The Competing Effect of Initial Crack Depth Versus Chemical Strengthening Parameters on Apparent Fracture Toughness of Sodium Aluminosilicate Glass,"The widespread use of sodium aluminosilicate glass in many engineering applications due to its mechanical and optical properties (transparency, dielectric, etc.), has become common in recent years. However, glass, a brittle material, has its vulnerability to fracture. Processes such as heat treatment (heat tempering) or chemical strengthening through ion-exchange have been used to create residual stress profiles on the glass, in a bid to improve its fracture strength. However, failure still occurs, which is mostly catastrophic and expensive to repair. Therefore understanding, predicting, and eventually improving the resistance to damage or fracture of chemically strengthened glass is important to designing new glasses that would be tougher while retaining their transparency. The relationship between the glass residual stress parameters such as the compressive stress (CS), depth of compression layer (DOL), and central tension (CT) versus apparent (effective) fracture toughness for different crack depth was investigated in this study using a Silicon Carbide particle blast plus ring-on-ring (RoR) test method. The results also showed that improving the fracture resistance of glass via chemical strengthening requires a proper combination of CS, DOL, and CT, which is particularly dependent on the initial/existing crack (flaw) depth. It was determined that for a damage event involving the introduction of a shallow crack depth, the criterion for optimal resistance to fracture, in terms of apparent fracture toughness, is weighted more towards a high CS, than deep DOL while for a deep flaw damage event, it is more weighted towards deep DOL, than a high CS. These results provide a valuable piece of information in the design of a more robust glass in engineering applications.",2012.04732v1 2021-04-07,Ultra-Thin Lubricant-Infused Vertical Graphene Nanoscaffolds for High-Performance Dropwise Condensation,"Lubricant-infused surfaces (LIS) are highly efficient in repelling water and constitute a very promising family of materials for condensation processes occurring in a broad range of energy applications. However, the performance of LIS in such processes is limited by the inherent thermal resistance imposed by the thickness of the lubricant and supporting surface structure, as well as by the gradual depletion of the lubricant over time. Here we present a remarkable, ultra-thin (~70 nm) and conductive LIS architecture, obtained by infusing lubricant into a vertically grown graphene nanoscaffold on copper. The ultra-thin nature of the scaffold, combined with the high in-plane thermal conductivity of graphene, drastically minimize earlier limitations, effectively doubling the heat transfer performance compared to a state-of-the-art CuO LIS surface. We show that the effect of the thermal resistance to the heat transfer performance of a LIS surface, although often overlooked, can be so detrimental that a simple nanostructured CuO surface can outperform a CuO LIS surface, despite film condensation on the former. The present vertical graphene LIS is also found to be resistant to lubricant depletion, maintaining stable dropwise condensation for at least ~7 hours with no significant change of advancing contact angle and contact angle hysteresis. The lubricant consumed by the vertical graphene LIS is 52.6% less than the existing state-of-the-art CuO LIS, making also the fabrication process more economical.",2104.03091v1 2023-07-24,Large negative magnetoresistance and pseudogap phase in superconducting A15-type La$_4$H$_{23}$,"High pressure plays a crucial role in the field of superconductivity. Compressed hydride superconductors are leaders in the race for a material that can conduct electricity without resistance at high or even room temperature. In the present work, we have discovered new lanthanum superhydride, cubic A15-type La$_4$H$_{23}$, with lower stabilization pressure compared to the reported $\textit{fcc}$ LaH$_{10}$. Superconducting La$_4$H$_{23}$ was obtained by laser heating of LaH$_3$ with ammonia borane at about 120 GPa. Transport measurements reveal the maximum critical temperature $\textit{T}$$_{C}$(onset) = 105 K and the critical field $\textit{H}$$_{C2}$(0) = 32 T at 118 GPa, as evidenced by the sharp drop of electrical resistance and the displacement of superconducting transitions in applied magnetic fields. Moreover, we provide evidence for unconventional transport associated with a pseudogap phase in La$_4$H$_{23}$ using pulsed magnetic fields up to 68 T. A large negative magnetoresistance in the non-superconducting state below 40 K, quasi $\textit{T}$-linear electrical resistance, and a sign-change of its temperature dependence mark the emergence of pseudogap in this hydride. Discovered lanthanum hydride is a new member of the A15 family of superconductors with $\textit{T}$$_C$ exceeding the boiling point of liquid nitrogen.",2307.13067v3 2019-07-04,Contact Engineering High Performance n-Type MoTe2 Transistors,"Semiconducting MoTe2 is one of the few two-dimensional (2D) materials with a moderate band gap, similar to silicon. However, this material remains under-explored for 2D electronics due to ambient instability and predominantly p-type Fermi level pinning at contacts. Here, we demonstrate unipolar n-type MoTe2 transistors with the highest performance to date, including high saturation current (>400 ${\mu}A/{\mu}m$ at 80 K and >200 ${\mu}A/{\mu}m$ at 300 K) and relatively low contact resistance (1.2 to 2 $k{\Omega}\cdot{\mu}m$ from 80 to 300 K), achieved with Ag contacts and AlOx encapsulation. We also investigate other contact metals, extracting their Schottky barrier heights using an analytic subthreshold model. High-resolution X-ray photoelectron spectroscopy reveals that interfacial metal-Te compounds dominate the contact resistance. Among the metals studied, Sc has the lowest work function but is the most reactive, which we counter by inserting monolayer h-BN between MoTe2 and Sc. These metal-insulator-semiconductor (MIS) contacts partly de-pin the metal Fermi level and lead to the smallest Schottky barrier for electron injection. Overall, this work improves our understanding of n-type contacts to 2D materials, an important advance for low-power electronics.",1907.02587v1 2011-03-11,Optimized fabrication of high quality La0.67Sr0.33MnO3 thin films considering all essential characteristics,"In this article, an overview of the fabrication and properties of high quality La0.67Sr0.33MnO3 (LSMO) thin films is given. A high quality LSMO film combines a smooth surface morphology with a large magnetization and a small residual resistivity, while avoiding precipitates and surface segregation. In literature, typically only a few of these issues are adressed. We therefore present a thorough characterization of our films, which were grown by pulsed laser deposition. The films were characterized with reflection high energy electron diffraction, atomic force microscopy, x-ray diffraction, magnetization and transport measurements, x-ray photoelectron spectroscopy and scanning transmission electron microscopy. The films have a saturation magnetization of 4.0 {\mu}B/Mn, a Curie temperature of 350 K and a residual resistivity of 60 {\mu}{\Omega}cm. These results indicate that high quality films, combining both large magnetization and small residual resistivity, were realized. A comparison between different samples presented in literature shows that focussing on a single property is insufficient for the optimization of the deposition process. For high quality films, all properties have to be adressed. For LSMO devices, the thin film quality is crucial for the device performance. Therefore, this research is important for the application of LSMO in devices.",1103.2267v1 2022-10-24,Nanomolding of Metastable Mo$_{4}$P$_{3}$,"Reduced dimensionality leads to emergent phenomena in quantum materials and there is a need for accelerated materials discovery of nanoscale quantum materials in reduced dimensions. Thermomechanical nanomolding is a rapid synthesis method that produces high quality single-crystalline quantum nanowires with controlled dimensions over wafer-scale sizes. Herein, we apply nanomolding to fabricate nanowires from bulk feedstock of MoP, a triple-point topological metal with extremely high conductivity that is promising for low-resistance interconnects. Surprisingly, we obtained single-crystalline Mo$_{4}$P$_{3}$ nanowires, a metastable phase at room temperature in atmospheric pressure. We thus demonstrate nanomolding can create metastable phases inaccessible by other nanomaterial syntheses and can explore a previously inaccessible synthesis space at high temperatures and pressures. Furthermore, our results suggest that the current understanding of interfacial solid diffusion for nanomolding is incomplete, providing opportunities to explore solid-state diffusion at high-pressure and high-temperature regimes in confined dimensions.",2210.13392v1 2024-02-02,Nano-ironing van der Waals Heterostructures Towards Electrically Controlled Quantum Dots,"Assembling two-dimensional van der Waals layered materials into heterostructures is an exciting development that sparked the discovery of rich correlated electronic phenomena and offers possibilities for designer device applications. However, resist residue from fabrication processes is a major limitation. Resulting disordered interfaces degrade device performance and mask underlying transport physics. Conventional cleaning processes are inefficient and can cause material and device damage. Here, we show that thermal scanning probe based cleaning can effectively eliminate resist residue to recover pristine material surfaces. Our technique is compatible at both the material- and device-level, and we demonstrate the significant improvement in the electrical performance of 2D WS2 transistors. We also demonstrate the cleaning of van der Waals heterostructures to achieve interfaces with low disorder. This enables the electrical formation and control of quantum dots that can be tuned from macroscopic current flow to the single-electron tunnelling regime. Such material processing advances are crucial for constructing high-quality vdW heterostructures that are important platforms for fundamental studies and building blocks for quantum and nano-electronics applications.",2402.01185v1 2024-02-13,Plasma-wall interaction in laser inertial fusion reactors: novel proposals for radiation tests of first wall materials,"Dry-wall laser inertial fusion (LIF) chambers will have to withstand strong bursts of fast charged particles which will deposit tens of kJ m$^{-2}$ and implant more than 10$^{18}$ particles m$^{-2}$ in a few microseconds at a repetition rate of some Hz. Large chamber dimensions and resistant plasma-facing materials must be combined to guarantee the chamber performance as long as possible under the expected threats: heating, fatigue, cracking, formation of defects, retention of light species, swelling and erosion. Current and novel radiation resistant materials for the first wall need to be validated under realistic conditions. However, at present there is a lack of facilities which can reproduce such ion environments. This contribution proposes the use of ultra-intense lasers and high-intense pulsed ion beams (HIPIB) to recreate the plasma conditions in LIF reactors. By target normal sheath acceleration, ultra-intense lasers can generate very short and energetic ion pulses with a spectral distribution similar to that of the inertial fusion ion bursts, suitable to validate fusion materials and to investigate the barely known propagation of those bursts through background plasmas/gases present in the reactor chamber. HIPIB technologies, initially developed for inertial fusion driver systems, provide huge intensity pulses which meet the irradiation conditions expected in the first wall of LIF chambers and thus can be used for the validation of materials too.",2402.10235v1 2002-03-25,Photo-response of the conductivity in functionalized pentacene compounds,"We report the first investigation of the photo-response of the conductivity of a new class of organic semiconductors based on functionalized pentacene. These materials form high quality single crystals that exhibit a thermally activated resistivity. Unlike pure pentacene, the functionalized derivatives are readily soluble in acetone, and can be evaporated or spin-cast as thin films for potential device applications. The electrical conductivity of the single crystal materials is noticeably sensitive to ambient light changes. The purpose, therefore, of the present study, is to determine the nature of the photo-response in terms of carrier activation vs. heating effects, and also to measure the dependence of the photo-response on photon energy. We describe a new method, involving the temperature dependent photo-response, which allows an unambiguous identification of the signature of heating effects in materials with a thermally activated conductivity. We find strong evidence that the photo-response in the materials investigated is predominantly a highly localized heating mechanism. Wavelength dependent studies of the photo-response reveal resonant features and cut-offs that indicate the photon energy absorption is related to the electronic structure of the material.",0203522v1 2016-04-19,Tuning the work function in transition metal oxides and their heterostructures,"The development of novel functional materials in experimental labs combined with computer-based compound simulation brings the vision of materials design on a microscopic scale continuously closer to reality. For many applications interface and surface phenomena rather than bulk properties are key. One of the most fundamental qualities of a material-vacuum interface is the energy required to transfer an electron across this boundary, i.e. the work function. It is a crucial parameter for numerous applications, including organic electronics, field electron emitters, and thermionic energy converters. Being generally very resistant to degradation at high temperatures, transition metal oxides present a promising materials class for such devices. We have performed a systematic study for perovskite oxides that provides reference values and, equally important, reports on materials trends and the tunability of work functions. Our results identify and classify dependencies of the work function on several parameters including specific surface termination, surface reconstructions, oxygen vacancies, and heterostructuring.",1604.05615v1 2020-04-15,Featureless adaptive optimization accelerates functional electronic materials design,"Electronic materials exhibiting phase transitions between metastable states (e.g., metal-insulator transition materials with abrupt electrical resistivity transformations) are challenging to decode. For these materials, conventional machine learning methods display limited predictive capability due to data scarcity and the absence of features impeding model training. In this article, we demonstrate a discovery strategy based on multi-objective Bayesian optimization to directly circumvent these bottlenecks by utilizing latent variable Gaussian processes combined with high-fidelity electronic structure calculations for validation in the chalcogenide lacunar spinel family. We directly and simultaneously learn phase stability and band gap tunability from chemical composition alone to efficiently discover all superior compositions on the design Pareto front. Previously unidentified electronic transitions also emerge from our featureless adaptive optimization engine. Our methodology readily generalizes to optimization of multiple properties, enabling co-design of complex multifunctional materials, especially where prior data is sparse.",2004.07365v2 2022-11-08,Extraordinary magnetometry -- a review on extraordinary magnetoresistance,"Extraordinary magnetoresistance (EMR) is a geometric magnetoresistance effect occurring in hybrid devices consisting of a high-mobility material joined by a metal. The change in resistance can exceed 107% at room temperature when a magnetic field of 5 T is applied. Magnetic field sensors based on EMR hold the potential formeasuring weak magnetic fields with an unprecedented sensitivity, yet, to date this potential is largely unmet. In this work, we provide an extensive review of the current state-of-the-art in EMR sensors with a focus on the hybrid device geometries, the constituent material properties and applications of EMR. We present a direct comparison of the best devices in literature across magnetoresistance, sensitivity and noise equivalent field for different materials and geometric designs. The compilation of studies collected in this review illustrates the extremely rich possibilities for tuning the magnetoresistive behavior varying the device geometry and material properties. In addition, we aim to improve the understanding of the EMR effect and its interplay with geometry and material properties. Finally, we discuss recent trends in the field and future perspectives for EMR.",2211.04308v1 2015-07-24,Measurements of the Rate Capability of Various Resistive Plate Chambers,"Resistive Plate Chambers (RPCs) exhibit a significant loss of efficiency for the detection of particles, when subjected to high particle fluxes. This rate limitation is related to the usually high resistivity of the resistive plates used in their construction. This paper reports on measurements of the performance of three different glass RPC designs featuring a different total resistance of the resistive plates. The measurements were performed with 120 GeV protons at varying beam intensities",1507.06968v2 2006-06-17,Elastomeric carbon nanotube circuits for local strain sensing,"We use elastomeric polydimethylsiloxane substrates to strain single-walled carbon nanotubes and modulate their electronic properties, with the aim of developing flexible materials that can sense local strain. We demonstrate micron-scale nanotube devices that can be cycled repeatedly through strains as high as 20% while providing reproducible local strain transduction by via the device resistance. We also compress individual nanotubes, and find they undergo an undulatory distortion with a characteristic spatial period of 100-200 nm. The observed period can be understood by the mechanical properties of nanotubes and the substrate in conjunction with continuum elasticity theory. These could potentially be used to create superlattices within individual nanotubes, enabling novel devices and applications.",0606463v1 2007-06-12,Very large spontaneous electric polarization in BiFeO3 single crystals at room temperature and its evolution under cycling fields,"Electric polarization loops are measured at room temperature on highly pure BiFeO3 single crystals synthesized by a flux growth method. Because the crystals have a high electrical resistivity, the resulting low leakage currents allow us to measure a large spontaneous polarization reaching 100 microC.cm^{-2}, a value never reported in the bulk. During electric cycling, the slow degradation of the material leads to an evolution of the hysteresis curves eventually preventing full saturation of the crystals.",0706.1681v1 2008-04-23,Giant Carrier Mobility in Single Crystals of FeSb2,"We report the giant carrier mobility in single crystals of FeSb2. Nonlinear field dependence of Hall resistivity is well described with the two-carrier model. Maximum mobility values in high mobility band reach ~10^5 cm^2/Vs at 8 K, and are ~10^2 cm^2/Vs at the room temperature. Our results point to a class of materials with promising potential for applications in solid state electronics.",0804.3625v1 2011-01-30,Thermodynamics of second phase conductive filaments,"We present a theory of second phase conductive filaments in phase transformable systems; applications include threshold switches, phase change memory, and shunting in thin film structures. We show that the average filament parameters can be described thermodynamically. In agreement with the published data, the predicted filament current voltage characteristics exhibit negative differential resistance vanishing at high currents where the current density becomes a bulk material property. Our description is extendible to filament transients and allows for efficient numerical simulation.",1101.5737v2 2012-08-30,Calculation of thermal parameters of SiGe microbolometers,"The thermal parameters of a SiGe microbolometer were calculated using numerical modeling. The calculated thermal conduction and thermal response time are in good agreement with the values found experimentally and range between 2x10$^-7$ and 7x10$^-8$ W/K and 1.5 and 4.5 ms, respectively. High sensitivity of microbolometer is achieved due to optimization of the thermal response time and thermal conduction by fitting the geometry of supporting heat-removing legs or by selection of a suitable material providing boundary thermal resistance higher than 8x10$^-3$ cm$^2$K/W at the SiGe interface.",1208.6147v1 2022-02-22,Superconductivity and weak anti-localization in nodal-line semimetal SnTaS_2,"Topological semimetals with superconducting properties provide an emergent platform to explore the properties of topological superconductors. We report magnetization, and magneto-transport measurements on high quality single crystals of transition metal dichalcogenide SnTaS2. It is a nodal line semimetal with superconducting transition below Tc = 2.9 K. Moderate anisotropy (3.1) is observed in upper critical fields along H||c and H||ab plane. In the normal state we observe large magneto-resistance and weak anti-localization effect that provide unambiguous confirmation of topological features in SnTaS2. Therefore, genuine topological characteristics can be studied in this material, particularly with regard to microscopic origin of order parameter symmetry.",2202.10711v1 2020-05-07,HVDC Surface Flashover in Compressed Air for Various Dielectrics,"This study measures the voltage at which flashover occurs in compressed air for a variety of dielectric materials and lengths in a uniform field for DC voltages up to 100 kV. Statistical time lag is recorded and characterized, displaying a roughly exponential dependence on breakdown voltage. Of the materials tested, acrylic is observed to be the most resistant to flashover. These data are intended to facilitate the design of compressed-air insulated high voltage systems as an alternative to SF6 insulated systems.",2006.12615v2 2023-07-30,Non-Equilibrium Nature of Fracture Determines the Crack Paths,"A high-fidelity neural network-based force field, NN-F$^{3}$, is developed to cover the strain states up to material failure and the non-equilibrium, intermediate nature of fracture. Simulations of fracture in 2D crystals using NN-F$^{3}$ reveal spatial complexities from lattice-scale kinks to sample-scale patterns. We find that the fracture resistance cannot be quantified by the energy densities of relaxed edges as in the literature. Instead, the fracture patterns, critical stress intensity factors at the kinks, and energy densities of edges in the intermediate, unrelaxed states offer reasonable measures for the fracture toughness and its anisotropy.",2307.16126v1 2004-09-30,Scaling theory of magneto-resistance in disordered local moment ferromagnets,"We present a scaling theory of magneto-transport in Anderson-localized disordered ferromagnets. Within our framework a pronounced magnetic-field-sensitive resistance peak emerges naturally for temperatures near the magnetic phase transition. We find that the resistance anomaly is a direct consequence of the change in localization length caused by the magnetic transition. For increasing values of the external magnetic field, the resistance peak is gradually depleted and pushed towards higher temperatures. Our results are in good agreement with magneto-resistance measurements on a variety of disordered magnets.",0410003v2 2009-02-08,Pulse width controlled resistivity switching at room temperature in Bi0.8Sr0.2MnO3,"We report pulsed as well as direct current/voltage induced electroresistance in Bi0.8Sr0.2MnO3 at room temperature. It is shown that bi-level and multi-level resistivity switching can be induced by a sequence of pulses of varying pulse width at fixed voltage amplitude. Resistivity increases abruptly (= 55 % at 300 K) upon reducing pulse width from 100 ms to 25 ms for a fixed electric field (E = 2 V/cm2) of 200 ms pulse period. The resistivity switching is accompanied by a periodic change in temperature which alone can not explain the magnitude of the resistivity change.",0902.1281v1 2010-01-05,Mechanism for bipolar resistive switching in transition metal oxides,"We introduce a model that accounts for the bipolar resistive switching phenomenom observed in transition metal oxides. It qualitatively describes the electric field-enhanced migration of oxygen vacancies at the nano-scale. The numerical study of the model predicts that strong electric fields develop in the highly resistive dielectric-electrode interfaces, leading to a spatially inhomogeneous oxygen vacancies distribution and a concomitant resistive switching effect. The theoretical results qualitatively reproduce non-trivial resistance hysteresis experiments that we also report, providing key validation to our model.",1001.0703v1 2011-05-19,Nonvolatile bipolar resistive switching in Au/BiFeO3/Pt,"Nonvolatile bipolar resistive switching has been observed in an Au/BiFeO3/Pt structure, where a Schottky contact and a quasi-Ohmic contact were formed at the Au/BiFeO3 and BiFeO3/Pt interface, respectively. By changing the polarity of the external voltage, the Au/BiFeO3/Pt is switched between two stable resistance states without an electroforming process. The resistance ratio is larger than two orders of magnitude. The resistive switching is understood by the electric field - induced carriers trapping and detrapping, which changes the depletion layer thickness at the Au/BiFeO3 interface.",1105.3827v1 2011-07-30,Polaronic transport in the ferromagnetic phase of Gd1-xCaxBaCo2O5.53,"Temperature dependent electrical resistivity and thermopower measurements were carried out on Gd1-xCaxBaCo2O5.53 with x varying between 0 and 0.25. Ca subsitution leads to the incorporation of holes (Co4+) into the system that leads to a reduction in resistivity and a stabilisation of the ferromagnetic phase at low temperatures. The temperature dependence of resistivity and thermopower are markedly different in the Ca doped sample, with a dramatic reduction in the resistivity, as compared to that in the pristine sample. The variation in both the resistivity and thermopower with temperature is explained in terms of the transport of polarons in the ferromagnetic phase of Ca doped system.",1108.0059v1 2017-06-20,Scaling of the Hall effects beyond the quantum resistance threshold in oxidized CoFeB,"The ordinary and the extraordinary Hall effects were studied in gradually oxidized amorphous CoFeB ferromagnets over six orders of resistivity from the metallic to the strongly insulating regime. Polarity of the extraordinary Hall effect reverses, and the amplitude of both the ordinary and the extraordinary Hall effects increases quadratically with resistivity when resistance exceeds the quantum resistance threshold. The absolute value of the extraordinary Hall effect scales linearly with the ordinary one in the entire range over eight orders of magnitude between the metallic and the insulating states. The behavior differs qualitatively and quantitatively from theoretically predicted and experimentally known in other materials.",1706.06392v1 2016-03-11,Measurement of the $B_{1g}$ and $B_{2g}$ components of the elastoresistivity tensor for tetragonal materials via transverse resistivity configurations,"The elastoresistivity tensor $m_{ij,kl}$ relates changes in resistivity to strains experienced by a material. As a fourth-rank tensor, it contains considerably more information about the material than the simpler (second-rank) resistivity tensor; in particular, for a tetragonal material, the $B_{1g}$ and $B_{2g}$ components of the elastoresistivity tensor ($m_{xx,xx}-m_{xx,yy}$ and $2m_{xy,xy}$, respectively) can be related to its nematic susceptibility. Previous experimental probes of this quantity have focused exclusively on differential longitudinal elastoresistance measurements, which determine the induced resistivity anisotropy arising from anisotropic in-plane strain based on the difference of two longitudinal resistivity measurements. Here we describe a complementary technique based on \textit{transverse} elastoresistance measurements. This new approach is advantageous because it directly determines the strain-induced resistivity anisotropy from a single transverse measurement. To demonstrate the efficacy of this new experimental protocol, we present transverse elastoresistance measurements of the $2m_{xy,xy}$ elastoresistivity coefficient of BaFe$_2$As$_2$, a representative iron-pnictide that has previously been characterized via differential longitudinal elastoresistance measurements.",1603.03537v1 2017-04-13,Low temperature physical properties of Co-35Ni-20Mo-10Cr alloy MP35N,"Multiphase Co-35Ni-20Mo-10Cr alloy MP35N is a high strength alloy with excellent corrosion resistance. Its applications span chemical, medical, and food processing industries. Thanks to its high modulus and high strength, it found applications in reinforcement of ultra-high field pulsed magnets. Recently, it has also been considered for reinforcement in superconducting wires used in ultra-high field superconducting magnets. For these applications, accurate measurement of its physical properties at cryogenic temperatures is very important. In this paper, physical properties including electrical resistivity, specific heat, thermal conductivity, and magnetization of as-received and aged samples are measured from 2 to 300 K. The electrical resistivity of the aged sample is slightly higher than the as-received sample, both showing a weak linear temperature dependence in the entire range of 2 - 300 K. The measured specific heat Cp of 0.43 J/g-K at 295 K agrees with a theoretical prediction, but is significantly smaller than the values in the literature. The thermal conductivity between 2 and 300 K is in good agreement with the literature which is only available above 77 K. Magnetic property of MP35N changes significantly with aging. The as-received sample exhibits Curie paramagnetism with a Curie constant C = 0.175 K. While the aged sample contains small amounts of a ferromagnetic phase even at room temperature. The measured MP35N properties will be useful for the engineering design of pulsed magnets and superconducting magnets using MP35N as reinforcement.",1704.04275v1 2024-02-20,Molten Salt Flux Liquid Transport Method for Ultra Clean Single Crystals UTe2,"Various single crystal growth techniques are presented for the unconventional superconductor UTe2. The molten salt flux liquid transport (MSFLT) method is employed to grow high-quality and large single crystals, exhibiting a high residual resistivity ratio (RRR = 200-800). On the other hand, the Te self-flux and chemical vapor transport (CVT) method produces samples of lower quality. The MSFLT method is a hybrid approach that combines the molten salt flux (MSF) and CVT methods. One significant advantage is that the materials gradually crystallize at the relatively low temperature which is fixed during the main process. This might be crucial for preventing U deficiency and obtaining high-quality and large single crystals of UTe2. Many different single crystals obtained by different technique were characterized by resistivity, specific heat measurements. The superconducting transition temperature decreases with the residual resistivity, followed by the Abrikosov-Gor'kov pair breaking theory. The highest quality sample reaches Tc=2.1K. The residual gamma-value of specific heat for the highest quality sample is only 3 percents of the normal state gamma-value. The specific heat jump, Delta C/(gamma Tc) reaches about 2.7 for high quality samples, indicating a strong coupling superconductor. Furthermore, the magnetic susceptibility for the field along a-axis in a high quality single crystal does not show an up-turn behavior on cooling, which is consistent with the results of NMR Knight shift and muSR experiments.",2402.12740v2 2023-12-29,Bilayer Vanadium Dioxide Thin Film with Elevated Transition Temperatures and High Resistance Switching,"Despite widespread interest in the phase-change applications of vanadium dioxide (VO$_2$), the fabrication of high-quality VO$_2$ thin films with elevated transition temperatures (TIMT) and high Insulator-Metal-Transition resistance switching still remains a challenge. This study introduces a two-step atmospheric oxidation approach to fabricate bilayer VO$_{2-x}$/VO$_2$ films on a c-plane sapphire substrate. To quantify the impact of the VO$_2$ buffer layer, a single-layer VO$_2$ film of the same thickness was also fabricated. The bilayer VO$_{2-x}$/VO$_2$ films wherein the top VO$_{2-x}$ film was under-oxidized demonstrated an elevation in TIMT reaching ~97 $^\circ$C, one of the highest reported to date for VO$_2$ films and is achieved in a doping-free manner. Our results also reveal a one-order increase in resistance switching, with the optimum bilayer VO$_2$/VO$_2$ film exhibiting ~3.6 orders of switching from 25 $^\circ$C to 110 $^\circ$C, compared to the optimum single-layer VO$_2$ reference film. This is accompanied by a one-order decrease in the on-state resistance in its metallic phase. The elevation in TIMT, coupled with increased strain extracted from the XRD characterization of the bilayer film, suggests the possibility of compressive strain along the c-axis. These VO$_{2-x}$/VO$_2$ films also demonstrate a significant change in the slope of their resistance vs temperature curves contrary to the conventional smooth transition. This feature was ascribed to the rutile/monoclinic quasi-heterostructure formed due to the top VO$_{2-x}$ film having a reduced TIMT. Our findings carry significant implications for both the lucid fabrication of VO$_2$ thin film devices as well as the study of phase transitions in correlated oxides.",2312.17437v1 2024-01-31,Spark Plasma Sintering for high-speed diffusion welding of the ultrafine grained near-a Ti-5Al-2V alloy with high strength and corrosion resistance for nuclear engineering,"The paper demonstrates the prospects of Spark Plasma Sintering (SPS) for the high-speed diffusion welding of the high-strength ultrafine-grained (UFG) near-a Ti-5Al-2V alloy. The effect of increased diffusion welding intensity in the UFG Ti alloys is discussed also. The welds of the UFG near-a-Ti-5Al-2V alloy obtained by SPS are featured by high density, strength, and corrosion resistance. The rate of weld sealing in the UFG alloys has been shown to depend on the heating rate non-monotonously (with a pronounced maximum). At the stage of continuous heating and isothermic holding, the kinetics of the weld sealing was found to be determined by the exponential creep rate, the intensity of which in the coarse-grained (CG) alloys is limited by the diffusion rate in the crystal lattice whereas in the UFG alloys it is limited by the grain boundary diffusion rate.",2401.17718v1 2018-01-29,Memristor properties of high temperature superconductors,"The review of studies on memristive properties or effect of resistive switchings in four classes of high temperature superconductors is presented in order to reveal functional properties of HTSCs which become apparent in the effects under discussion, prospects of usage of high temperature superconductors based memristors in applications and search for new mechanisms of strongly correlated nature to realize new generation memristors. The properties are: undergoing metal insulator transition at oxygen doping, transport anisotropy, existence of charge reservoirs through which doping of conductive copper oxygen layers is carried out. These are the main functional properties of HTSCs which permit to use them in memristors. By the example of study of bipolar effect of resistive switching in high temperature superconductors based heterojunctions it is shown how one can form memristor structures based on high temperature superconductors using their functional properties.",1801.09428v1 2016-03-07,Prediction of a Two-dimensional Phosphorus Nitride Monolayer,"Today, 2D semiconductor materials have been extended into the nitrogen group: phosphorene, arsenene, antimonene and even nitrogene. Motivated by them, based upon first-principles density functional calculations, we propose a new two-dimensional phosphorus nitride (PN) structure that is stable well above the room temperature, due to its extremely high cohesive energy. Unlike phosphorene, PN structure is resistant to high temperature oxidation. The structure is predicted to be a semiconductor with a wide, indirect band gap of 2.64 eV. More interestingly, the phosphorus nitride monolayer experiences an indirect-to-direct band-gap transition at a relatively small tensile strain. Such dramatic transformation in the electronic structure combined with structural stability and oxidation resistance at high temperature could pave the way for exciting innovations in high-speed ultrathin transistors, power electronic modules, ultra-high efficiency LEDs and semiconductor lasers.",1603.01957v2 2023-04-12,Crack-free high composition (>35%) thick (>30 nm) barrier AlGaN/AlN/GaN HEMT on sapphire with record low sheet resistance,"In this article, high composition (>35%) thick (>30 nm) barrier AlGaN/AlN/GaN HEMT structure grown on a sapphire substrate with ultra-low sheet resistivity (<250 \Omega / \Box ) is reported. Optimization of growth conditions, such as reduced growth rate, low carbon incorporation, and thickness optimization of different epitaxial layers allowed to grow a crack-free high composition and thick AlGaN barrier layer HEMT structure. A significantly high two-dimensional electron gas (2DEG) density of 1.46 \times 10^{13} cm^{-2} with a room temperature mobility of 1710 cm^{2}/V.s is obtained by Hall measurement using the Van-Der-Pauw method. These state-of-the-art results show great potential for high-power Ga-polar HEMT design on the sapphire substrate.",2304.05593v1 2015-02-06,Long-term stability of phase-separated Half-Heusler compounds,"Half-Heusler (HH) compounds have shown high Figure of merits up to 1.5. The key to these high thermoelectric efficiencies is an intrinsic phase separation, which occurs in multicomponent Half-Heusler compounds and leads to an significantly reduction of the thermal conductivity. For commercial applications, compatible n- and p-type materials are essential and their thermal stability under operating conditions, e.g. for an automotive up to 873 K, needs to be guaranteed. For the first time, the long-term stability of n- and p-type HH materials is proved. We investigated HH materials based on the Ti0.3Zr0.35Hf0.35NiSn-system after 500 cycles (1700 h) from 373 to 873 K. Both compounds exhibit a maximum Seebeck coefficient of S around 210 muV/K and an intrinsic phase separation into two HH phases. The dendritic microstructure is temperature resistant and maintained the low thermal conductivity values (kappa less than 4 W/Km). Our results emphasize that phase-separated HH compounds are suitable low cost materials and can lead to enhanced thermoelectric efficiencies beyond the set benchmark for industrial applications.",1502.01828v1 2020-08-12,Helium effects and bubbles formation in irradiated Ti3SiC2,"Ti3SiC2 is a potential structural material for nuclear reactor applications. However, He irradiation effects in this material are not well understood, especially at high temperatures. Here, we compare the effects of He irradiation in Ti3SiC2 at room temperature (RT) and at 750 {\deg}C. Irradiation at 750 {\deg}C was found to lead to extremely elongated He bubbles that are concentrated in the nano-laminate layers of Ti3SiC2, whereas the overall crystal structure of the material remained intact. In contrast, at RT, the layered structure was significantly damaged and highly disordered after irradiation. Our study reveals that at elevated temperatures, the unique structure of Ti3SiC2 can accommodate large amounts of He atoms in the nano-laminate layer, without compromising the structural stability of the material. The structure and the mechanical tests results show that the irradiation induced swelling and hardening at 750 {\deg}C are much smaller than those at RT. These results indicate that Ti3SiC2 has an excellent resistance to accumulation of radiation-induced He impurities and that it has a considerable tolerance to irradiation-induced degradation of mechanical properties at high temperatures.",2008.05468v1 2023-09-05,"Control of Mechanical and Fracture Properties in Two-phase Materials Reinforced by Continuous, Irregular Networks","Composites with high strength and high fracture resistance are desirable for structural and protective applications. Most composites, however, suffer from poor damage tolerance and are prone to unpredictable fractures. Understanding the behavior of materials with an irregular reinforcement phase offers fundamental guidelines for tailoring their performance. Here, we study the fracture nucleation and propagation in two phase composites, as a function of the topology of their irregular microstructures. We use a stochastic algorithm to design the polymeric reinforcing network, achieving independent control of topology and geometry of the microstructure. By tuning the local connectivity of isodense tiles and their assembly into larger structures, we tailor the mechanical and fracture properties of the architected composites, at the local and global scale. Finally, combining different reinforcing networks into a spatially determined meso-scale assembly, we demonstrate how the spatial propagation of fractures in architected composite materials can be designed and controlled a priori.",2309.01888v1 2020-01-21,"Mechanical behavior, enhanced dc resistivity, energy band gap and high temperature magnetic properties of Y-substituted Mg-Zn ferrites","We report the synthesis of Y-substituted Mg-Zn ferrites using conventional standard ceramic technique. XRD patterns confirm the single phase cubic spinel structure up to x = 0.03 and appearance of a secondary phase of YFeO3for higher Y contents. FESEM images depict the distribution of grains and EDS spectra confirmed the absence of any unwanted element. Completion of solid state reaction and formation of spinel structure has been revealed from FTIR spectra. The FTIR data along with lattice constant, bulk density and porosity were further used to calculate the stiffness constant (Cij), elastic constant and Debye temperatures. Mechanical stability of all studied compositions is confirmed from Cij using Born stability conditions. Brittleness and isotropic nature are also confirmed using Poisson ratio and anisotropy constants, respectively. The enhancement of dc electrical resistivity with Y content is observed. The energy band gap (increased with Y contents) is found in good agreement with dc electrical resistivity. Ferrimagnetic to paramagnetic phase change has been observed from the field dependent high temperature magnetization curves. The magnetic moments and saturation magnetization were found to be decreased with increasing temperature. The Curie temperature (Tc) has been measured from temperature dependent magnetic moment (M-T) and initial permeability and found to be in good agreement with each other. Decrease in Tc with Y content is due to redistribution of cations and weakening of the exchange coupling constant. The magnetic phase transition has been analyzed by Arrott plot and found to have second order phase transition. The dc resistivity endorses the prepared ferrites are suitable for high frequency and high temperature magnetic device applications as well.",2001.07313v1 2023-01-07,Impact of Severe Plastic Deformation on Kinetics and Thermodynamics of Hydrogen Storage in Magnesium and Its Alloys,"Magnesium and its alloys are the most investigated materials for solid-state hydrogen storage in the form of metal hydrides, but there are still unresolved problems with the kinetics and thermodynamics of hydrogenation and dehydrogenation of this group of materials. Severe plastic deformation (SPD) methods, such as equal-channel angular pressing (ECAP), high-pressure torsion (HPT), intensive rolling and fast forging, have been widely used to enhance the activation, air resistance, and hydrogenation/dehydrogenation kinetics of Mg-based hydrogen storage materials by introducing ultrafine/nanoscale grains and crystal lattice defects. These severely deformed materials, particularly in the presence of alloying additives or second-phase nanoparticles, can show not only fast hydrogen absorption/desorption kinetics but also good cycling stability. It was shown that some materials that are apparently inert to hydrogen can absorb hydrogen after SPD processing. Moreover, the SPD methods were effectively used for hydrogen binding-energy engineering and synthesizing new magnesium alloys with low thermodynamic stability for reversible low/room-temperature hydrogen storage, such as nanoglasses, high-entropy alloys, and metastable phases including the high-pressure {\gamma}-MgH2 polymorph. This article reviews recent advances in the development of Mg-based hydrogen storage materials by SPD processing and discusses their potential in future applications.",2301.05009v1 2021-07-26,Massive electrons and unconventional room-temperature superconductivity in superhydrides,"The search for room-temperature superconducting materials has been at the center of modern research for decades. The recent discovery of high-temperature superconductivity, under extreme pressure in hydrogen-rich materials, is a tremendous achievement in this research front. This discovery offers a route in the search for room temperature superconductivity at ambient pressure. The superconductivity of these hydrogen-rich materials was confirmed by the observation of zero-resistance, isotope effects, effect of magnetic field, and other standard properties. However, some of the experimental features were puzzling as they were not consistent with the known superconductivity theories. These debatable features have lead to a series of recent publications downplaying the existence of superconductivity in these superhydrides. Here we propose a concept of massive electrons under pressure and successfully explain all non-standard experimental observations. Our massive electron concept explains the large effective mass of the quasiparticles, the reason for the high critical temperatures for moderate electron-phonon couplings, and a 3-5 orders of magnitude larger conductivity causing a narrow resistivity broadening at the transition in the presence of magnetic field. We anticipate our findings will lead to a new directions and tweaks in current research in the search for ambient-pressure, room-temperature superconductors.",2107.12255v1 2010-04-21,Superconductor-insulator quantum phase transition,"The current understanding of the superconductor-insulator transition is discussed level by level in a cyclic spiral-like manner. At the first level, physical phenomena and processes are discussed which, while of no formal relevance to the topic of transitions, are important for their implementation and observation; these include superconductivity in low electron density materials, transport and magnetoresistance in superconducting island films and in highly resistive granular materials with superconducting grains, and the Berezinskii-Kosterlitz-Thouless transition. The second level discusses and summarizes results from various microscopic approaches to the problem, whether based on the Bardeen-Cooper-Schrieffer theory (the disorder-induced reduction in the superconducting transition temperature; the key role of Coulomb blockade in high-resistance granular superconductors; superconducting fluctuations in a strong magnetic field) or on the theory of the Bose-Einstein condensation. A special discussion is given to phenomenological scaling theories. Experimental investigations, primarily transport measurements, make the contents of the third level and are for convenience classified by the type of material used (ultrathin films, variable composition materials, high-temperature superconductors, superconductor-poor metal transitions). As a separate topic, data on nonlinear phenomena near the superconductor-insulator transition are presented. At the final, summarizing, level the basic aspects of the problem are enumerated again to identify where further research is needed and how this research can be carried out. Some relatively new results, potentially of key importance in resolving the remaining problems, are also discussed.",1004.3761v1 2016-03-30,"Butterfly Magnetoresistance, Quasi-2D Dirac Fermi Surfaces, and a Topological Phase Transition in ZrSiS","Magnetoresistance (MR), the change of a material's electrical resistance in response to an applied magnetic field, is a technologically important property that has been the topic of intense study for more than a quarter century. Here we report the observation of an unusual ""butterfly"" shaped titanic angular magnetoresistance (AMR) in the non-magnetic, Dirac material, ZrSiS. The MR is large and positive, reaching nearly 1.8 x 10^5 percent at 9 T and 2 K at an angle of 45o between the applied current (along the a-axis) and the applied field (90o is H parallel to the c-axis). Approaching 90o, a ""dip"" is seen in the AMR which can be traced to an angle dependent deviation from the H^2 law. By analyzing the SdH oscillations at different angles, we find that ZrSiS has a combination of 2D and 3D Dirac pockets comprising its Fermi surface and that the anomalous transport behavior coincides with a topological phase transition whose robust signature is evident despite transport contributions from other parts of the Fermi surface. We also find that as a function of angle, the temperature dependent resistivity in high field displays a broad peak-like behavior, unlike any known Dirac/Weyl material. The combination of very high mobility carriers and multiple Fermi surfaces in ZrSiS allow for large bulk property changes to occur as a function of angle between applied fields makes it a promising platform to study the physics stemming from the coexistence of 2D and 3D Dirac electrons.",1603.09318v2 2020-08-27,Large-Scale and Robust Multifunctional Vertically-Aligned MoS$_2$ Photo-Memristors,"Memristive devices have drawn considerable research attention due to their potential applications in non-volatile memory and neuromorphic computing. The combination of resistive switching devices with light-responsive materials is considered a novel way to integrate optical information with electrical circuitry. On the other hand, 2D materials have attracted substantial consideration thank to their unique crystal structure, as reflected in their chemical and physical properties. Although not the major focus, van der Waals solids were proven to be potential candidates in memristive devices. In this scheme, the majority of the resistive switching devices were implemented on planar flakes, obtained by mechanical exfoliation. Here we utilize a facile and robust methodology to grow large-scale vertically aligned MoS$_2$ (VA-MoS$_2$) films on standard silicon substrates. Memristive devices with the structure silver/VA-MoS$_2$/Si are shown to have low set-ON voltages (<0.5V), large-retention times ($>2\times10^4$ s) and high thermal stability (up to 350 $^\circ$C). The proposed memristive device also exhibits long term potentiation / depression (LTP/LTD) and photo-active memory states. The large-scale fabrication, together with the low operating voltages, high thermal stability, light-responsive behaviour and long-term potentiation/depression, makes this approach very appealing for real-life non-volatile memory applications.",2008.11950v1 2002-08-15,High Ferromagnetic Transition Temperature (172K) in Mn delta-doped GaAs with p-type Selective Doping,"We have found high ferromagnetic transition temperature in Mn delta-doped GaAs-based heterostructures grown on GaAs(001) substrates by molecular beam epitaxy. A 0.3 ML Mn d-doped GaAs samples showed high resistivity at low temperature and did not show a ferromagnetic behavior. However, in a selectively doped heterostructure (Mn delta-doped GaAs / Be-doped AlGaAs), where holes were supplied from the Be-doped AlGaAs layer, clear ferromagnetic order was observed. The ferromagnetic transition temperature of the selectively doped heterostructure was as high as 172K with suitable low-temperature (LT) annealing treatment.",0208299v1 2013-10-30,"Large, high quality single-crystals of the new Topological Kondo Insulator, SmB6","SmB6 has recently been predicted to be a Topological Kondo Insulator, the first strongly correlated heavy fermion material to exhibit topological surface states. High quality crystals are necessary to investigate the topological properties of this material. Single crystal growth of the rare earth hexaboride, SmB6, has been carried out by the floating zone technique using a high power xenon arc lamp image furnace. Large, high quality single-crystals are obtained by this technique. The crystals produced by the floating zone technique are free of contamination from flux materials and have been characterised by resistivity and magnetisation measurements. These crystals are ideally suited for the investigation of both the surface and bulk properties of SmB6.",1310.8189v1 2019-11-05,Metal$/BaTiO_{3}/β-Ga_{2}O_{3}$ Dielectric Heterojunction Diode with 5.7 MV/cm Breakdown Field,"Wide and ultra-wide band gap semiconductors can provide excellent performance due to their high energy band gap, which leads to breakdown electric fields that are more than an order of magnitude higher than conventional silicon electronics. In materials where p-type doping is not available, achieving this high breakdown field in a vertical diode or transistor is very challenging. We propose and demonstrate the use of dielectric heterojunctions that use extreme permittivity materials to achieve high breakdown field in a unipolar device. We demonstrate the integration of a high permittivity material BaTiO3 with n-type $\beta$-Ga2O3 to enable 5.7 MV/cm average electric field and 7 MV/cm peak electric field at the device edge, while maintaining forward conduction with relatively low on-resistance and voltage loss. The proposed dielectric heterojunction could enable new design strategies to achieve theoretical device performance limits in wide and ultra-wide band gap semiconductors where bipolar doping is challenging.",1911.02068v1 2009-03-17,In search for the superconducting spin-switch: Magnetization induced resistance switching effects in La$_{0.67}$Sr$_{0.33}$MnO$_3$/YBa$_2$Cu$_3$O$_{7-δ}$ bi- and trilayers,"We have studied the influence of the magnetization on the superconducting transition temperature ($T_c$) in bi- and trilayers consisting of the half-metallic ferromagnet La$_{0.67}$Sr$_{0.33}$MnO$_3$ (LSMO) and the high-temperature superconductor YBa$_2$Cu$_3$O$_{7-\delta}$ (YBCO). We have made use of tilted epitaxial growth in order to achieve contacts between the two materials that are partly in the crystallographic $ab$-plane of the YBCO. As a result of uniaxial magnetic anisotropy in the tilted structures, we observe sharp magnetization switching behavior. At temperatures close to $T_c$, the magnetization switching induces resistance jumps in trilayers, resulting in a magnetization dependence of $T_c$. In bilayers, this switching effect can be observed as well, provided that the interface to the ferromagnetic layer is considerably rough. Our results indicate that the switching behavior arises from magnetic stray fields from the ferromagnetic layers that penetrate into the superconductor. A simple model describes the observed behavior well. We find no evidence that the switching behavior is caused by a so-called superconducting spin-switch, nor by accumulation of spin-polarized electrons. Observation of magnetic coupling of the ferromagnetic layers, through the superconductor, supports the idea of field induced resistance switching.",0903.2993v1 2016-12-13,Bad Metals from Fluctuating Density Waves,"Bad metals have a large resistivity without being strongly disordered. In many bad metals the Drude peak moves away from zero frequency as the resistivity becomes large at increasing temperatures. We catalogue the position and width of the `displaced Drude peak' in the observed optical conductivity of several families of bad metals, showing that $\omega_\text{peak} \sim \Delta \omega \sim k_BT/\hbar$. This is the same quantum critical timescale that underpins the $T$-linear dc resistivity of many of these materials. We provide a unified theoretical description of the optical and dc transport properties of bad metals in terms of the hydrodynamics of short range quantum critical fluctuations of incommensurate density wave order. Within hydrodynamics, pinned translational order is essential to obtain the nonzero frequency peak.",1612.04381v5 2017-03-11,On the isotope effect in compressed superconducting H$_\textrm{3}$S and D$_\textrm{3}$S,"A maximum superconductive transition temperature $T_\textrm{C}$ = 203.5 K has recently been reported for a sample of the binary compound tri-hydrogen sulfide (H$_\textrm{3}$S) prepared at high pressure and with room temperature annealing. Measurements of $T_\textrm{C}$ for H$_\textrm{3}$S and its deuterium counterpart D$_\textrm{3}$S have suggested a mass isotope effect exponent ${\alpha}$ with anomalous enhancements for reduced applied pressures. While widely cited for evidence of phonon-based superconductivity, the measured $T_\textrm{C}$ is shown to exhibit important dependences on the quality and character of the H$_\textrm{3}$S and D$_\textrm{3}$S materials under study; examination of resistance versus temperature data shows that variations in $T_\textrm{C}$ and apparent ${\alpha}$ are strongly correlated with residual resistance ratio, indicative of sensitivity to metallic order. Correlations also extend to the fractional widths of the superconducting transitions. Using resistance data to quantify and compensate for the evident materials differences between H$_\textrm{3}$S and D$_\textrm{3}$S samples, a value of ${\alpha}$ = 0.043 $\pm$ 0.140 is obtained. Thus, when corrected for the varying levels of disorder, the experimental upper limit ($\leq$0.183) lies well below ${\alpha}$ derived in phonon-based theories.",1703.04034v1 2019-07-17,Quasi 2-D magnetism in the Kagome layer compound FeSn,"Single crystals of the single Kagome layer compound FeSn are investigated using x-ray and neutron scattering, magnetic susceptibility and magnetization, heat capacity, resistivity, Hall, Seebeck, thermal expansion, thermal conductivity measurements and density functional theory (DFT). FeSn is a planar antiferromagnet below TN = 365 K and exhibits ferromagnetic magnetic order within each Kagome layer. The in-plane magnetic susceptibility is sensitive to synthesis conditions. Resistivity, Hall and Seebeck results indicate multiple bands near the Fermi energy. The resistivity of FeSn is about 3 times lower for current along the stacking direction than in the plane, suggesting that transport and the bulk electronic structure of FeSn is not quasi 2D. FeSn is an excellent metal with Rho(300K)/Rho(2K) values about 100 in both directions. While the ordered state is antiferromagnetic, high temperature susceptibility measurements indicate a ferromagnetic Curie-Weiss temperature of 173 K, reflecting the strong in-plane ferromagnetic interactions. DFT calculations show a 3D electronic structure with the Dirac nodal lines along the K-H directions in the magnetic Brillouin zone about 0.3 eV below the Fermi energy, with the Dirac dispersions at the K points gapped by spin-orbit coupling except at the H point. The magnetism, however, is highly 2D with Jin-plane/Jout-of-plane = 10. The predicted spin-wave spectrum is presented.",1907.07719v1 2019-06-25,Spin-split band hybridization in graphene proximitized with $α$-RuCl$_3$ nanosheets,"Proximity effects induced in the 2D Dirac material graphene potentially open access to novel and intriguing physical phenomena. Thus far, the coupling between graphene and ferromagnetic insulators has been experimentally established. However, only very little is known about graphene's interaction with antiferromagnetic insulators. Here, we report a low temperature study of the electronic properties of high quality van der Waals heterostructures composed of a single graphene layer proximitized with $\alpha$-RuCl$_3$. The latter is known to become antiferromagnetically ordered below 10 K. Shubnikov de Haas oscillations in the longitudinal resistance together with Hall resistance measurements provide clear evidence for a band realignment that is accompanied by a transfer of electrons originally occupying the graphene's spin degenerate Dirac cones into $\alpha$-RuCl$_3$ band states with in-plane spin polarization. Left behind are holes in two separate Fermi pockets, only the dispersion of one of which is distorted near the Fermi energy due to spin selective hybridization with these spin polarized $\alpha$-RuCl$_3$ band states. This interpretation is supported by our DFT calculations. An unexpected damping of the quantum oscillations as well as a zero field resistance upturn close to the N$\'e$el temperature of $\alpha$-RuCl$_3$ suggests the onset of additional spin scattering due to spin fluctuations in the $\alpha$-RuCl$_3$.",1906.10405v1 2020-01-17,"A back-end, CMOS compatible ferroelectric Field Effect Transistor for synaptic weights","Neuromorphic computing architectures enable the dense co-location of memory and processing elements within a single circuit. This co-location removes the communication bottleneck of transferring data between separate memory and computing units as in standard von Neuman architectures for data-critical applications including machine learning. The essential building blocks of neuromorphic systems are non-volatile synaptic elements such as memristors. Key memristor properties include a suitable non-volatile resistance range, continuous linear resistance modulation and symmetric switching. In this work, we demonstrate voltage-controlled, symmetric and analog potentiation and depression of a ferroelectric Hf$_{57}$Zr$_{43}$O$_{2}$ (HZO) field effect transistor (FeFET) with good linearity. Our FeFET operates with a low writing energy (fJ) and fast programming time (40 ns). Retention measurements have been done over 4-bits depth with low noise (1%) in the tungsten oxide (WO$_{x}$) read out channel. By adjusting the channel thickness from 15nm to 8nm, the on/off ratio of the FeFET can be engineered from 1% to 200% with an on-resistance ideally >100 kOhm, depending on the channel geometry. The device concept is using earth-abundant materials, and is compatible with a back end of line (BEOL) integration into complementary metal-oxidesemiconductor (CMOS) processes. It has therefore a great potential for the fabrication of high density, large-scale integrated arrays of artificial analog synapses.",2001.06475v1 2020-05-16,Switching friction at a manganite surface using electric fields,"We report active control of the friction force at the contact between a nanoscale asperity and a La$_{0.55}$Ca$_{0.45}$MnO$_3$ (LCMO) thin film using electric fields. We use friction force microscopy under ultrahigh vacuum conditions to measure the friction force as we change the film resistive state by electric field-induced resistive switching. Friction forces are high in the insulating state and clearly change to lower values when the probed local region is switched to the conducting state. Upon switching back to an insulating state, the friction forces increase again. Thus, we demonstrate active control of friction without having to change the contact temperature or pressure. By comparing with measurements of friction at the metal-to-insulator transition and with the effect of applied voltage on adhesion, we rule out electronic excitations, electrostatic forces and changes in contact area as the reasons for the effect of resistive switching on friction. Instead, we argue that friction is limited by phonon relaxation times which are strongly coupled to the electronic degrees of freedom through distortions of the MnO6 octahedra. The concept of controlling friction forces by electric fields should be applicable to any materials where the field produces strong changes in phonon lifetimes.",2005.08949v1 2020-08-17,Enhancement of spin Hall conductivity in W-Ta alloy,"Generating pure spin currents via the spin Hall effect in heavy metals has been an active topic of research in the last decade. In order to reduce the energy required to efficiently switch neighbouring ferromagnetic layers for applications, one should not only increase the charge- to-spin conversion efficiency but also decrease the longitudinal resistivity of the heavy metal. In this work, we investigate the spin Hall conductivity in W_{1-x}Ta_{x} / CoFeB / MgO (x = 0 - 0.2) using spin torque ferromagnetic resonance measurements. Alloying W with Ta leads to a factor of two change in both the damping-like effective spin Hall angle (from - 0.15 to - 0.3) and longitudinal resistivity (60 - 120 {\mu}W cm). At 11% Ta concentration, a remarkably high spin Hall angle value of - 0.3 is achieved with a low longitudinal resistivity 100 {\mu}W cm, which could lead to a very low power consumption for this W-based alloy. This work demonstrates sputter-deposited W-Ta alloys could be a promising material for power-efficient spin current generation.",2008.07572v1 2020-12-23,"Resistivity, Hall effect, and anisotropic superconducting coherence lengths of HgBa$_2$CaCu$_2$O$_{6+δ}$ thin films with different morphology","Thin films of the high-temperature superconductor HgBa$_2$CaCu$_2$O$_{6+\delta}$ have been prepared on SrTiO$_3$ substrates by pulsed-laser deposition of precursor films and subsequent annealing in mercury-vapor atmosphere. The microstructural properties of such films can vary considerably and have been analyzed by x-ray diffraction and atomic force microscopy. Whereas the resistivity is significantly enhanced in samples with coarse-grained structure, the Hall effect shows little variation. This disparity is discussed based on models for transport properties in granular materials. We find that, despite of the morphological variation, all samples have similar superconducting properties. The critical temperatures $T_c \sim 121.2$ K $\dots 122.0$ K, resistivity, and Hall data indicate that the samples are optimally doped. The analyses of superconducting order parameter fluctuations in zero and finite magnetic fields yield the in-plane $\xi_{ab}(0) \sim 2.3$ nm $\dots 2.8$ nm and out-of-plane $\xi_{c}(0) \sim 0.17$ nm $ \dots 0.24$ nm Ginzburg-Landau coherence lengths at zero temperature. Hall measurements provide estimates of carrier scattering defects in the normal state and vortex pinning properties in the superconducting state inside the grains.",2012.12539v1 2021-05-03,Fingerprints of quantum criticality in locally resolved transport,"Understanding electrical transport in strange metals, including the seeming universality of Planckian $T$-linear resistivity, remains a longstanding challenge in condensed matter physics. We propose that local imaging techniques, such as nitrogen vacancy center magnetometry, can locally identify signatures of quantum critical response which are invisible in measurements of a bulk electrical resistivity. As an illustrative example, we use a minimal holographic model for a strange metal in two spatial dimensions to predict how electrical current will flow in regimes dominated by quantum critical dynamics on the Planckian length scale. We describe the crossover between quantum critical transport and hydrodynamic transport (including Ohmic regimes), both in charge neutral and finite density systems. We compare our holographic predictions to experiments on charge neutral graphene, finding quantitative agreement with available data; we suggest further experiments which may determine the relevance of our framework to transport on Planckian scales in this material. More broadly, we propose that locally imaged transport be used to test the universality (or lack thereof) of microscopic dynamics in the diverse set of quantum materials exhibiting $T$-linear resistivity.",2105.01075v4 2022-06-16,Size-Dependent Grain Boundary Scattering in Topological Semimetals,"We assess the viability of topological semimetals for application in advanced interconnect technology, where conductor size is on the order of a few nanometers and grain boundaries are expected to be prevalent. We investigate the electron transport properties and grain boundary scattering in thin films of the topological semimetals CoSi and CoGe using first-principles calculations combined with the Non-Equilibrium Green's Function (NEGF) technique. Unlike conventional interconnect metals like Cu and Al, we find that CoSi and CoGe conduct primarily through topologically-protected surface states in thin film structures even in the presence of grain boundaries. The area-normalized resistance decreases with decreasing film thickness for CoSi and CoGe thin films both with and without grain boundaries; a trend opposite to that of the conventional metals Cu and Al. The surface-dominated transport mechanisms in thin films of topological semimetals with grain boundaries demonstrates a fundamentally new paradigm of the classical resistivity size-effect, and suggests that these materials may be promising candidates for applications as nano-interconnects where high electrical resistivity acts as a major bottleneck limiting semiconductor device performance.",2206.08214v2 2023-03-06,Thermal hysteretic behavior and negative magnetoresistance in an unusual charge-density-wave material EuTe4,"EuTe4 is a newly-discovered van der Waals material exhibiting a novel charge-density wave (CDW) with a large thermal hysteresis in the resistivity and CDW gap. In this work, we systematically study the electronic structure and transport properties of EuTe4 using high-resolution angle-resolved photoemission spectroscopy (ARPES), magnetoresistance measurements, and scanning tunneling microscopy (STM). We observe a CDW gap of about 200 meV at low temperatures that persists up to 400 K, suggesting that the CDW transition occurs at a much higher temperature. We observe a large thermal hysteretic behavior of the ARPES intensity near the Fermi level, consistent with the resistivity measurement. The hysteresis in the resistivity measurement does not change under a magnetic field up to 7 T, excluding the thermal magnetic hysteresis mechanism. Instead, the surface topography measured with STM shows surface domains with different CDW trimerization directions, which may be important for the thermal hysteretic behavior of EuTe4. Interestingly, we observe a large negative magnetoresistance at low temperatures that can be associated with the canting of magnetically ordered Eu spins. Our work shed light on the understanding of magnetic, transport, and electronic properties of EuTe4.",2303.02848v1 2023-05-10,Doubling of the superconducting transition temperature in ultra-clean wafer-scale aluminum nanofilms,"Superconducting properties of thin films can be vastly different from those of bulk materials. Seminal work has shown the critical temperature Tc of elemental superconductors decreases with decreasing film thickness when the normal-state sheet resistance is lower than the quantum resistance h/(4e2). Sporadic examples on disordered films, however, hinted an enhancement in Tc although, structural and strain characterization was not possible since samples were prepared on a cold substrate in situ. To clarify the role of reduced dimensionality and disorder on the superconducting properties of thin films we employed molecular beam epitaxy to grow wafer-scale high-quality aluminum (Al) nanofilms with normal-state sheet resistance at least 20 times lower than h/(4e2) and investigated their electronic and structural properties ex situ. Defying general expectations, Tc increases with decreasing Al film thickness, reaching 2.4 K for 3.5-nm-thick Al film grown on GaAs: twice that of bulk Al (1.2 K). DFT calculations indicate surface phonon softening impacts superconductivity in pure ultra-thin films, offering a new route for materials engineering in two dimensions.",2305.06084v1 1999-06-17,Anomalous c-axis charge dynamics in copper oxide materials,"Within the t-J model, the c-axis charge dynamics of the copper oxide materials in the underdoped and optimally doped regimes is studied by considering the incoherent interlayer hopping. It is shown that the c-axis charge dynamics is mainly governed by the scattering from the in-plane fluctuation. In the optimally doped regime, the c-axis resistivity is a linear in temperatures, and shows the metallic-like behavior for all temperatures, while the c-axis resistivity in the underdoped regime is characterized by a crossover from the high temperature metallic-like behavior to the low temperature semiconducting-like behavior, which are consistent with experiments and numerical simulations.",9906260v2 2001-07-04,Crystal Growth and Characterization of Doped CZT Crystals,"Cd1-xZnxTe crystals with x in the range of 0.1-0.2 were grown by the high-pressure vertical Bridgman method from pre-synthesized CZT. Resistive graphite heaters were used to control the temperature profiles within the furnaces, and an argon overpressure was used to reduce the cadmium loss. The crystals were doped with either Al, Ni, In, Ga, Ge or Sn. The doping was carried out by three different ways: 1) by adding of the pure metals during growth runs; 2) by adding of the tellurides of the metals during growth runs; or 3) by inserting of the metal tellurides during synthesis of the starting CZT material. Some of the growth process parameters were also varied. The as-grown CZT ingots had diameters of either 15 or 38 mm. The influence of the doping on CZT properties, particularly the conductivity type and specific electrical resistivity, will be discussed. Energy spectra from alpha particles (U-233, Ra-226, and U-233+Pu-239+Pu-238) and from different gamma sources (Cs-137, Co-60, Co-57, Am-241) will be reported.",0107081v1 2007-05-29,Sliding charge density wave in manganites,"The so-called stripe phase of the manganites is an important example of the complex behaviour of metal oxides, and has long been interpreted as the localisation of charge at atomic sites. Here, we demonstrate via resistance measurements on La_{0.50}Ca_{0.50}MnO_3 that this state is in fact a prototypical charge density wave (CDW) which undergoes collective transport. Dramatic resistance hysteresis effects and broadband noise properties are observed, both of which are typical of sliding CDW systems. Moreover, the high levels of disorder typical of manganites result in behaviour similar to that of well-known disordered CDW materials. Our discovery that the manganite superstructure is a CDW shows that unusual transport and structural properties do not require exotic physics, but can emerge when a well-understood phase (the CDW) coexists with disorder.",0705.4310v2 2009-02-23,Superconductivity at 22.3 K in SrFe2-xIrxAs2,"By substituting the Fe with the 5d-transition metal Ir in SrFe2As2, we have successfully synthesized the superconductor SrFe2-xIrxAs2 with Tc = 22.3 K at x = 0.5. X-ray diffraction indicates that the material has formed the ThCr2Si2-type structure with a space group I4/mmm. The temperature dependence of resistivity and dc magnetization both reveal sharp superconducting transitions at around 22 K. An estimate on the diamagnetization signal reveals a high Meissner shielding volume. Interestingly, the normal state resistivity exhibits a roughly linear behavior up to 300 K. The superconducting transitions at different magnetic fields were also measured yielding a slope of -dHc2/dT = 3.8 T/K near Tc. Using the Werthamer-Helfand-Hohenberg (WHH) formula, the upper critical field at zero K is found to be about 58 T. Counting the possible number of electrons doped into the system in SrFe2-xIrxAs2, we argue that the superconductivity in the Ir-doped system is different from the Co-doped case, which should add more ingredients to the underlying physics of the iron pnictide superconductors.",0902.3957v2 2009-09-07,SiC Graphene Suitable For Quantum Hall Resistance Metrology,"We report the first observation of the quantum Hall effect in epitaxial graphene. The result described in the submitted manuscript fills the yawning gap in the understanding of the electronic properties of this truly remarkable material and demonstrate suitability of the silicon carbide technology for manufactiring large area high quality graphene. Having found the quantum Hall effect in several devices produced on distant parts of a single large-area wafer, we can confirm that material synthesized on the Si-terminated face of SiC promises a suitable platform for the implementations of quantum resistance metrology at elevated temperatures and, in the longer term, opens bright prospects for scalable electronics based on graphene.",0909.1193v1 2010-07-07,Unusual Resistance Hysteresis in n-Layer Graphene Field Effect Transistors Fabricated on Ferroelectric Pb(Zr_0.2Ti_0.8)O_3,"We have fabricated n-layer graphene field effect transistors on epitaxial ferroelectric Pb(Zr_0.2Ti_0.8)O_3 (PZT) thin films. At low gate voltages, PZT behaves as a high-k dielectric with k up to 100. An unusual resistance hysteresis occurs in gate sweeps at high voltages, with its direction opposite to that expected from the polarization switching of PZT. The relaxation of the metastable state is thermally activated, with an activation barrier of 50-110 meV and a time constant of 6 hours at 300 K. We attribute its origin to the slow dissociation/recombination dynamics of water molecules adsorbed at the graphene-PZT interface. This robust hysteresis can potentially be used to construct graphene-ferroelectric hybrid memory devices.",1007.1240v1 2011-01-15,Theory of anomalous Hall effect for type-II high-Tc and conventional superconductors,"The anomalous Hall effect for type-II superconductors is investigated by random walk theorem. It is shown that the origin of Hall anomaly is induced by the thermally activated vortex bundle flow (TAVBF) over the directional-dependent energy barrier formed by the Magus force, random collective pinning force, and strong pinning force inside the vortex bundles. The directional-dependent potential barrier of the vortex bundles renormalizes the Hall and longitudinal resistivities strongly. Under the framework of present theory, it is also shown that the Hall anomaly is universal for type-II superconductors, either high- or conventional as well as bulk materials or thin films. The conditions for Hall anomaly and reentry phenomenon are derived, the Hall and longitudinal resistivities as well as Hall angle for type-II superconducting films and bulk materials versus temperature and applied magnetic field are calculated. All the results are in agreement with the experiments.",1101.2943v1 2011-12-08,Circuit Modeling of Tunneling Real-Space Transfer Transistors: Toward Terahertz Frequency Operation,"High frequency operation of tunneling real-space transfer transistor (TRSTT) in the negative differential resistance (NDR) regime is assessed by calculating the device common source unity current gain frequency (fT) range with a small signal equivalent circuit model including tunneling. Our circuit model is based on an In0.2Ga0.8As and delta-doped GaAs dual channel structure with various gate lengths. The calculated TRSTT fT agrees very well with experimental data, limiting factor being the resistance of the delta-doped GaAs layer. By optimizing the gate dimensions and channel materials, we find fT in the NDR region approaches terahertz range, which anticipates potential use of TRSTT as terahertz sources.",1112.1980v1 2013-01-24,Spin transport parameters in metallic multilayers determined by ferromagnetic resonance measurements of spin pumping,"We measured spin transport in nonferromagnetic (NM) metallic multilayers from the contribution to damping due to spin pumping from a ferromagnetic Co90Fe10 thin film. The multilayer stack consisted of NM1/NM2/Co90Fe10(2 nm)/NM2/NM3 with varying NM materials and thicknesses. Using conventional theory for one dimensional diffusive spin transport in metals, we show that the effective damping due to spin pumping can be strongly affected by the spin transport properties of each NM in the multilayer, which permits the use of damping measurements to accurately determine the spin transport properties of the various NM layers in the full five-layer stack. We find that due to its high electrical resistivity, amorphous Ta is a poor spin conductor, in spite of a short spin-diffusion length of 1.0 nm, and that Pt is an excellent spin conductor by virtue of its low electrical resistivity and a spin diffusion length of only 0.5 nm. Spin Hall effect measurements may have underestimated the spin Hall angle in Pt by assuming a much longer spin diffusion length.",1301.5861v1 2014-11-01,Manipulating electronic states at oxide interfaces using focused micro X-rays from standard lab-sources,"Recently, x-ray illumination, using synchrotron radiation, has been used to manipulate defects, stimulate self-organization and to probe their structure. Here we explore a method of defect-engineering low-dimensional systems using focused laboratory-scale X-ray sources. We demonstrate an irreversible change in the conducting properties of the 2-dimensional electron gas at the interface between the complex oxide materials LaAlO3 and SrTiO3 by X-ray irradiation. The electrical resistance is monitored during exposure as the irradiated regions are driven into a high resistance state. Our results suggest attention shall be paid on electronic structure modification in X-ray spectroscopic studies and highlight large-area defect manipulation and direct device patterning as possible new fields of application for focused laboratory X-ray sources.",1411.0177v1 2015-01-13,Phase-change memory function of correlated electrons in organic conductors,"Phase-change memory (PCM), a promising candidate for next-generation non-volatile memories, exploits quenched glassy and thermodynamically stable crystalline states as reversibly switchable state variables. We demonstrate PCM functions emerging from a charge-configuration degree of freedom in strongly correlated electron systems. Non-volatile reversible switching between a high-resistivity charge-crystalline (or charge-ordered) state and a low-resistivity quenched state, charge glass, is achieved experimentally via heat pulses supplied by optical or electrical means in organic conductors $\theta$-(BEDT-TTF)$_2$$X$. Switching that is one order of magnitude faster is observed in another isostructural material that requires faster cooling to kinetically avoid charge crystallization, indicating that the material's critical cooling rate can be useful guidelines for pursuing a faster correlated-electron PCM function.",1501.02873v2 2015-01-15,Optimizing the Optical and Electrical Properties of Graphene Ink Thin Films by Laser-annealing,"We demonstrate a facile fabrication technique for graphene-based transparent conductive films. Highly flat and uniform graphene films are obtained through the incorporation of an efficient laser annealing technique with one-time drop casting of high-concentration graphene ink. The resulting thin films are uniform and exhibit a transparency of more than 85% at 550 nm and a sheet resistance of about 30 k{\Omega}/sq. These values constitute an increase of 45% in transparency, a reduction of surface roughness by a factor of four and a decrease of 70% in sheet resistance compared to unannealed films.",1501.03843v1 2015-02-18,The Role of Transport Agents in MoS2 Single Crystals,"We report resistivity, thermoelectric power and thermal conductivity of MoS2 single crystals prepared by chemical vapour transport (CVT) method using I2, Br2 and TeCl4 as transport agents. The material presents low-lying donor and acceptor levels, which dominate the in-plane charge transport. Intercalates into the Van der Waals gap strongly influence the inter-plane resistivity. Thermoelectric power displays the characteristics of strong electron-phonon interaction. Detailed theoretical model of thermal conductivity reveals the presence of high number of defects in the MoS2 structure. We show that these defects are inherent to CVT growth method, coming mostly from the transport agent molecules inclusion as identified by Total Reflection X-ray Fluorescence analysis (TXRF) and in-beam activation analysis (IBAA).",1502.05161v1 2015-08-20,Transport Conductivity of Graphene at RF and Microwave Frequencies,"We measure graphene coplanar waveguides from direct current (DC) to 13.5GHz and show that the apparent resistance (in the presence of parasitic impedances) has an quadratic frequency dependence, but the intrinsic conductivity (without the influence of parasitic impedances) is frequency-independent. Consequently, in our devices the real part of the complex alternating current conductivity is the same as the DC value and the imaginary part~0. The graphene channel is modelled as a parallel resistive-capacitive network with a frequency dependence identical to that of the Drude conductivity with momentum relaxation time~2.1ps, highlighting the influence of alternating current (AC) electron transport on the electromagnetic properties of graphene. This can lead to optimized design of high-speed analogue field-effect transistors, mixers, frequency doublers, low-noise amplifiers and radiation detectors.",1508.04984v1 2016-08-17,Nanocomposite si-c-n coatings,"Coatings of ternary nanocomposite Si-C-N ceramic coatings have shown newer and improved mechanical and functional properties over the coarser and monolithic coatings. Properties like high hardness, wear resistance, oxidation resistance, tunable band gap and chemical inertness have been observed for Si-C-N which makes its potential for numerous applications. Although lot of research has taken place in Si-C-N coatings, proper understanding of the effect of different parameters on the coating properties are still not resolved. The changes occurring in fraction of Si, C and N and the phases forming in the coatings with variation in deposition conditions require investigations. This research paper gives a systematic study of the role of different deposition parameters like substrate temperature, pressure, power on the nucleation and growth, structure, microstructural bonding and mechanical properties of the film deposited by magnetron sputtering which adds significantly to the fundamental knowledge of nanocomposite Si-C-N coatings as well as its applications.",1608.05667v1 2016-12-21,Correlation between battery material performance and cooperative electron-phonon interaction in LiCo$_y$Mn$_{2-y}$O$_{4}$,"Understanding the basic physics related to archetypal lithium battery material (such as LiCo$_y$Mn$_{2-y}$O$_{4}$) is of considerable interest and is expected to aid designing of cathodes of high capacity. The relation between electrochemical performance, activated-transport parameters, thermal expansion, and cooperativity of electron-phonon-interaction distortions in LiCo$_y$Mn$_{2-y}$O$_{4}$ is investigated. The first order cooperative-normal-mode transition, detected through coefficient of thermal expansion, is found to disappear at a critical doping ($y \sim 0.16$); interestingly, for $y \gtrsim 0.16$ the resistivity does not change much with doping and the electrochemical capacity becomes constant over repeated cycling. The critical doping $y \sim 0.16$ results in breakdown of the network of cooperative/coherent normal-mode distortions; this leads to vanishing of the first-order transition, establishment of hopping channels with lower resistance, and enhancing lithiation and delithiation of the battery, thereby minimizing electrochemical capacity fading.",1612.07092v1 2018-05-07,High-temperature thermoelectric properties of half-Heusler phases Er$_{1-x}$Ho$_x$NiSb,"Polycrystalline samples of Er$_{1-x}$Ho$_x$NiSb ($x$ = 0, 0.2, 0.3, 0.5, 0.7, 0.8, 1) were characterized by means of x-ray powder diffraction (XRD), scanning electron microscopy (SEM), and optical metallography. The results proved the formation of half-Heusler alloys in the entire composition range. Their electrical transport properties (resistivity, thermoelectric power) were studied in the temperature interval 350-1000 K. The measured electrical resistivity spanned between 5 and 25 $\mu \Omega$m. The maximum thermopower of 50-65 $\mu$V/K was observed at temperatures 500-650 K. Replacing Ho for Er resulted in a non-monotonous variation of the thermoelectric power factor ($PF = S^2/\rho$). The largest $PF$ of 4.6 $\mu$WcmK$^{-2}$ was found at 660 K for Er$_{0.5}$Ho$_{0.5}$NiSb. This value is distinctly larger than PF determined for the terminal phases ErNiSb and HoNiSb.",1805.02435v1 2018-05-16,Magnetic properties of single crystalline itinerant ferromagnet AlFe2B2,"Single crystals of AlFe$_{2}$B$_{2}$ have been grown using the self flux growth method and then measured the structural properties, temperature and field dependent magnetization, and temperature dependent electrical resistivity at ambient as well as high pressure. The Curie temperature of AlFe$_{2}$B$_{2}$ is determined to be $274$~K. The measured saturation magnetization and the effective moment for paramagnetic Fe-ion indicate the itinerant nature of the magnetism with a Rhode-Wohlfarth ratio $ \frac{M_{C}}{M_{sat}}\approx 1.14$. Temperature dependent resistivity measurements under hydrostatic pressure shows that transition temperature \textit{T$_C$} is suppressed down to 255 K for $p = 2.24$~GPa pressure with a suppression rate of $\sim -8.9$~K/GPa. The anisotropy fields and magnetocrystalline anisotropy constants are in reasonable agreement with density functional theory calculations.",1805.06373v1 2019-09-29,Structural and electrical properties of ceramic Li-ion conductors based on Li$_{1.3}$Al$_{0.3}$Ti$_{1.7}$(PO$_4$)$_3$-LiF,"The work presents the investigations of Li1.3Al0.3Ti1.7(PO4)3-xLiF Li-ion conducting ceramics with 0 < x < 0.3 by means of X-ray diffractometry (XRD), 7Li, 19F, 27Al and 31P Magic Angle Spinning Nuclear Magnetic Resonance (MAS NMR) spectroscopy, thermogravimetry (TG), scanning electron microscopy (SEM), impedance spectroscopy (IS) and density method. It has been shown that the total ionic conductivity of both as-prepared and ceramic Li1.3Al0.3Ti1.7(PO4)3 is low due to a grain boundary phase exhibiting high electrical resistance. This phase consists mainly of berlinite crystalline phase as well as some amorphous phase containing Al3+ ions. The electrically resistant phases of the grain boundary decompose during sintering with LiF additive. The processes leading to microstructure changes and their effect on the ionic properties of the materials are discussed in the frame of the brick layer model (BLM). The highest total ionic conductivity at room temperature was measured for LATP-0.1LiF ceramic sintered at 800{\deg}C and was equal to {\sigma}tot = 1.1 x 10-4 Scm-1.",1909.13291v2 2017-03-19,A thermodynamic analysis of the spider silk and the importance of complexity,"The spider silk is one of the most interesting bio-materials investigated in the last years. One of the main reasons that brought scientists to study this organized system is its high level of resistance if compared to other artificial materials characterized by higher density. Subsequently, researchers discovered that the spider silk is a complex system formed by different kinds of proteins, organized (or disorganized) to guarantee the required resistance, which is function of the final application and of the environmental conditions. Some spider species are able to make different silks, up to twelve, having a composition that seems to be function of the final use (i.e. dragline web, capture web, etc). The aim of this paper is to analyze the properties of the spider silk by means of a thermodynamic approach, taking advantage of the well-known theories applied to polymers, and to try to underline and develop some intriguing considerations. Moreover, this study can be taken as an example to introduce and discuss the importance of the concept of optionality and of the anti-fragile systems proposed by N. N. Thaleb in his book ""Antifragile: Things that gain from disorder"".",1703.06497v1 2019-07-31,Large spin Hall magnetoresistance in antiferromagnetic α-Fe2O3/Pt heterostructures,"We investigate the spin Hall magnetoresistance (SMR) at room temperature in thin film heterostructures of antiferromagnetic, insulating, (0001)-oriented alpha-Fe2O3 (hematite) and Pt. We measure their longitudinal and transverse resistivities while rotating an applied magnetic field of up to 17T in three orthogonal planes. For out-of-plane magnetotransport measurements, we find indications for a multidomain antiferromagnetic configuration whenever the field is aligned along the film normal. For in-plane field rotations, we clearly observe a sinusoidal resistivity oscillation characteristic for the SMR due to a coherent rotation of the Neel vector. The maximum SMR amplitude of 0.25% is, surprisingly, twice as high as for prototypical ferrimagnetic Y3Fe5O12/Pt heterostructures. The SMR effect saturates at much smaller magnetic fields than in comparable antiferromagnets, making the alpha-Fe2O3/Pt system particularly interesting for room-temperature antiferromagnetic spintronic applications.",1907.13393v4 2020-09-16,Properties and influence of microstructure and crystal defects in Fe$_2$VAl modified by laser surface remelting,"Laser surface remelting can be used to manipulate the microstructure of cast material. Here, we present a detailed analysis of the microstructure of Fe$_2$VAl following laser surface remelting. Within the melt pool, elongated grains grow nearly epitaxially from the heat-affected zone. These grains are separated by low-angle grain boundaries with 1{\deg}-5{\deg} misorientations. Segregation of vanadium, carbon, and nitrogen at grain boundaries and dislocations is observed using atom probe tomography. The local electrical resistivity was measured by an in-situ four-point-probe technique. A smaller increase in electrical resistivity is observed at these low-angle grain boundaries compared to high-angle grain boundaries in a cast sample. This indicates that grain boundary engineering could potentially be used to manipulate thermoelectric properties.",2009.07685v2 2016-03-18,"Electronic Structure, Phase Stability and Resistivity of Hybrid Hexagonal C$_x$(BN)$_{1-x}$ Two-dimensional Nanomaterial: A First-principles Study","We use density functional theory based first-principles method to investigate the bandstructure and phase stability in the laterally grown hexagonal C$_x$(BN)$_{1-x}$, two-dimensional Graphene and $h$-BN hybrid nanomaterials, which were synthesized by experimental groups recently (Liu $et al$, Nature Nanotech, 8, 119 (2013)). Our detail electronic structure calculations on such materials, with both armchair and zigzag interfaces between the Graphene and $ h$-BN domains, indicate that the band-gap decreases non-monotonically with the concentration of Carbon. The calculated bandstructure shows the onset of Dirac cone like features near the band-gap at high Carbon concentration ($x \sim 0.8$). From the calculated energy of formation, the phase stability of C$_x$(BN)$_{1-x}$ was studied using a regular solution model and the system was found to be in the ordered phase below a few thousand Kelvin. Furthermore, using the Boltzmann transport theory we calculate the electrical resistivity from the bandstrcture of C$_x$(BN)$_{1-x}$ at different temperature ($T$), which shows a linear behaviour when plotted in the logarithmic scale against $T^{-1}$, as observed experimentally",1603.05780v1 2017-08-25,Ballistic geometric resistance resonances in a single surface of a topological insulator,"Transport in topological matter has shown a variety of novel phenomena over the last decade. Although numerous transport studies have been conducted on three-dimensional topological insulators (3D-TIs), study of ballistic motion and thus exploration of potential landscapes on a hundred nanometer scale is for the prevalent TI materials almost impossible due to their low carrier mobility. Therefore it is unknown whether helical Dirac electrons in TIs, bound to interfaces between topologically distinct materials, can be manipulated on the nanometer scale by local gates or locally etched regions. Here we impose a submicron periodic potential onto a single surface of Dirac electrons in high mobility strained mercury telluride (HgTe), which is a strong TI. Pronounced geometric resistance resonances constitute the first observation of a ballistic effect in 3D-TIs.",1708.07766v1 2018-08-22,Evidence for Undoped Weyl Semimetal Charge Transport in $Y_{2}Ir_{2}O_{7}$,"Weyl fermions scattering from a random Coulomb potential are predicted to exhibit resistivity versus temperature $\rho \space \alpha \space T^{-4}$ in a single particle model. Here we show that, in closed environment-grown polycrystalline samples of $Y_{2}Ir_{2}O_{7}$, $\rho = \rho_{0} T^{-4}$ over four orders of magnitude in $\rho$. While the measured prefactor, $\rho_{0}$, is obtained from the model using reasonable materials parameters, the $T^{-4}$ behavior extends far beyond the model's range of applicability. In particular, the behavior extends into the low-temperature, high-resistivity region where the Ioffe-Regel parameter, $k_{T} \ell \ll 2\pi$. Strong on-site Coulomb correlations, instrumental for predicting a Weyl semimetal state in $Y_{2}Ir_{2}O_{7}$, are the possible origin of such ""bad"" Weyl semimetal behavior.",1808.07583v4 2019-04-07,Restoration of long range order of Na ions in $Na_xCoO_2$ at high temperatures by sodium site doping,"We have systematically investigated the $Na_xCoO_2$ system doped with Cu, Y, Sn, W, Au and Bi for $x$ = 0:5; 0:75 and 1.00 using density functional theory. Sn, W, and Bi always substitute a Co while Au always substitutes a Na regardless of Na concentration. However, for Cu and Y, the substitution site depends on Na concentration. When compared to the available experimental data, we find that thermoelectric performance is enhanced when the dopants substitute a Na site. In this case, surprisingly, resistivity decreases despite the reduced hole concentration caused by carrier recombination. We propose improved carrier mobility to be the cause of observed reduced resistivity.",1904.03644v1 2019-08-07,Fast response of pulsed laser deposited Zinc ferrite thin film as a chemo-resistive gas sensor,"Thin films of ZnFe2O4 deposited by pulsed laser technique are here demonstrated as one of the interesting materials for sensing of ethanol. The response transients were fitted well to one-site Langmuir adsorption model. Activation energies for (I) adsorption and reaction of ethanol and (II) desorption (i.e. recovery process) of ethanol from zinc ferrite thin film surface were obtained on the basis of this model. In this paper, we showed the effect of operating temperature and gas-concentration on the response time of thin film sensor materials. At the operating temperature 340oC, the ZnFe2O4 thin film showed high (84%) as well as immediate response to 500 ppm of ethanol, with its resistance being saturated within ~12 seconds, which stands far superior to the response time of nano crystalline powders. Those films were also observed to have a good repeatability of their sensor response, thus representing a major step towards low-cost large-scale production of this class of devices.",1908.02780v1 2012-06-18,GdN Nanoisland-Based GaN Tunnel Junctions,"We show that GdN nanoislands can enhance inter-band tunneling in GaN PN junctions by several orders of magnitude, enabling low optical absorption low-resistance tunnel junctions (specific resistivity 1.3 X 10-3 {\Omega}-cm2) for various optoelectronic applications. We exploit the ability to overgrow high quality GaN over GdN nanoislands to create new nanoscale heterostructure designs that are not feasible in planar epitaxy. GdN nanoisland assisted inter-band tunneling was found to enhance tunneling in both of the polar orientations of GaN. Tunnel injection of holes was confirmed by low temperature operation of GaN p-n junction with a tunneling contact layer, showing strong electroluminescence down to 20K. The availability of tunnel junctions with negligible absorption could not only improve the efficiency of existing optoelectronic devices significantly, but also enable new electronic and optical devices based on wide band gap materials.",1206.3810v3 2015-07-01,Itinerant Antiferromagnetism in FeMnP0.8Si0.2 Single Crystals,"Compounds based on the Fe2P structure have continued to attract interest because of the interplay between itinerant and localized magnetism in a non-centrosymmetric crystal structure, and because of the recent developments of these materials for magnetocaloric applications. Here we report the growth and characterization of mm size single crystals of FeMnP0.8Si0.2. Single crystal x-ray diffraction, magnetization, resistivity, Hall and heat capacity data are reported. Surprisingly, the crystals exhibit itinerant antiferromagnetic order below 158 K with no hint of ferromagnetic behavior in the magnetization curves and with the spins ordered primarily in the ab plane. The room temperature resistivity is close to the Ioffe-Regel limit for a metal. Single crystal x-ray diffraction indicates a strong preference for Mn to occupy the larger pyramidal 3g site. The cation site preference in the as-grown crystals and the antiferromagnetism are not changed after high temperature anneals and a rapid quench to room temperature.",1507.00275v1 2019-01-22,S-type Negative Differential Resistance in Semiconducting Transition-Metal Dichalcogenides,"Current-controlled (also known as ""S-type"") negative differential resistance (NDR) is of crucial importance to many emerging applications including neuromorphic computing and high-density memristors integration. However, the experimental realization of S-type NDR based on conventional mechanisms poses demanding requirements on materials, which greatly limits their potential applications. Here, we experimentally identify that semiconducting transition metal dichalcogenides (TMDs) can host a bipolar S-type NDR devices. Theoretical simulations indicate that the origin of the NDR in these devices arises from a thermal feedback mechanism. Furthermore, we demonstrate the potential applications of TMDs based S-type NDR device in signal processing and neuromorphic electronics.",1901.07161v1 2020-12-30,High Current Density in Monolayer MoS$_2$ Doped by AlO$_x$,"Semiconductors require stable doping for applications in transistors, optoelectronics, and thermoelectrics. However, this has been challenging for two-dimensional (2D) materials, where existing approaches are either incompatible with conventional semiconductor processing or introduce time-dependent, hysteretic behavior. Here we show that low temperature (< 200$^\circ$ C) sub-stoichiometric AlO$_x$ provides a stable n-doping layer for monolayer MoS$_2$, compatible with circuit integration. This approach achieves carrier densities > 2x10$^{13}$ 1/cm$^2$, sheet resistance as low as ~7 kOhm/sq, and good contact resistance ~480 Ohm.um in transistors from monolayer MoS$_2$ grown by chemical vapor deposition. We also reach record current density of nearly 700 uA/um (>110 MA/cm$^2$) in this three-atom-thick semiconductor while preserving transistor on/off current ratio > $10^6$. The maximum current is ultimately limited by self-heating and could exceed 1 mA/um with better device heat sinking. With their 0.1 nA/um off-current, such doped MoS$_2$ devices approach several low-power transistor metrics required by the international technology roadmap",2012.15350v1 2021-06-09,Maximizing Spin-Orbit Torque Generated by the Spin Hall Effect of Pt,"Efficient generation of spin-orbit torques (SOTs) is central for the exciting field of spin-orbitronics. Platinum, the archetypal spin Hall material, has the potential to be an outstanding provider for spin-orbit torques due to its giant spin Hall conductivity, low resistivity, high stabilities, and the ability to be compatible with CMOS circuits. However, pure clean-limit Pt with low resistivity still provides a low damping-like spin-orbit torque efficiency, which limits its practical applications. The efficiency of spin-orbit torque in Pt-based magnetic heterostructures can be improved considerably by increasing the spin Hall ratio of Pt and spin transmissivity of the interfaces. Here we reviews recent advances in understanding the physics of spin current generation, interfacial spin transport, and the metrology of spin-orbit torques, and summarize progress towards the goal of Pt-based spin-orbit torque memories and logic that are fast, efficient, reliable, scalable, and non-volatile.",2106.04992v2 2021-08-12,Revisiting the Reduction of Thermal Conductivity in Nano- to Micro-Grained Bismuth Telluride: The Importance of Grain-Boundary Thermal Resistance,"Nanograined bulk alloys based on bismuth telluride (Bi2Te3) are the dominant materials for room-temperature thermoelectric applications. In numerous studies, existing bulk phonon mean free path (MFP) spectra predicted by atomistic simulations suggest sub-100 nm grain sizes are necessary to reduce the lattice thermal conductivity by decreasing phonon MFPs. This is in contrast with available experimental data, where a remarkable thermal conductivity reduction is observed even for micro-grained Bi2Te3 samples. In this work, first-principles phonon MFPs along both the in-plane and cross-plane directions are re-computed for bulk Bi2Te3. These phonon MFPs can explain new and existing experimental data on flake-like Bi2Te3 nanostructures with various thicknesses. For polycrystalline Bi2Te3-based materials, a better explanation of the experimental data requires further consideration of the grain-boundary thermal resistance that can largely suppress the transport of high-frequency optical phonons.",2108.05972v1 2022-12-02,Electric modulation of the Fermi arc spin transport via three-terminal configuration in the topological semimetal nanowires,"Spin momentum locking is a key feature of the topological surface state, which plays an important role in spintronics. The electrical detection of current-induced spin polarization protected by the spin momentum locking in non-magnetic systems provides a new platform for developing spintronics while previous studies were mostly based on magnetic materials. In this study, the spin transport measurement of Dirac semimetal Cd3As2 was studied by the three-terminal geometry, and a hysteresis loop signal with high resistance and low resistance state was observed. The hysteresis was reversed by reversing the current direction, which illustrates the spin-momentum locking feature of Cd3As2. Furthermore, we realized the on-off states of the spin signals through electric modulation of the Fermi arc via the three-terminal configuration, which enables the great potential of Cd3As2 in spin field-effect transistors.",2212.01072v1 2023-08-02,Observation of zero resistance above 100$^\circ$ K in Pb$_{10-x}$Cu$_x$(PO$_4$)$_6$O,"Room-temperature superconductivity has always been regarded as the ultimate goal in the fields of solid-state physics and materials science, with its realization holding revolutionary significance, capable of triggering significant changes in energy transmission and storage. However, achieving it poses various challenges. Recent research revealed that material Pb$_{10-x}$Cu$_x$(PO$_4$)$_6$O displays room-temperature superconductivity under atmospheric pressure, sparking global interest in further exploration. Here, we utilized solid-phase synthesis to obtain a polycrystalline sample of Pb$_{10-x}$Cu$_x$(PO$_4$)$_6$O. X-ray diffraction confirmed its structural consistency with referenced literature. Zero resistance, which is important evidence for superconductivity, was observed above 100$^\circ$ K under ambient pressure in our experiment. Our finding indicates that Pb$_{10-x}$Cu$_x$(PO$_4$)$_6$O is a possible candidate for searching high-temperature superconductors.",2308.01192v1 2024-04-13,Solution-Processed Inks with Fillers of NbS$_3$ Quasi-One-Dimensional Charge-Density-Wave Material,"We report on the solution processing and testing of electronic ink comprised of quasi-one-dimensional NbS$_3$ charge-density-wave fillers. The ink was prepared by liquid-phase exfoliation of NbS$_3$ crystals into high-aspect ratio quasi-1D fillers dispersed in a mixture of isopropyl alcohol and ethylene glycol solution. The results of the electrical measurements of two-terminal electronic test structures printed on silicon substrates reveal resistance anomalies in the temperature range of ~330 K to 370 K. It was found that the changes in the temperature-dependent resistive characteristics of the test structures originate from the charge-density-wave phase transition of individual NbS$_3$ fillers. The latter confirms that the exfoliated NbS$_3$ fillers preserve their intrinsic charge-density-wave quantum condensate states and can undergo phase transitions above room temperature even after chemical exfoliation processes and printing. These results are important for developing ""quantum inks"" with charge-density-wave fillers for the increased functionality of future solution-processed electronics.",2404.09038v1 2024-02-16,Cycling on rough roads: A model for resistance and vibration,"Minimising opposing forces is a matter of interest to most cyclists. These forces arise from passage through air (""drag"") and interaction with the road surface (""resistance""). Recent work recognises that resistance forces arise not only from the deformation of the tyre (""rolling resistance"") but also from irregularities in the road surface (""roughness resistance""), which lead to power dissipation in the body of the rider through vibration. The latter effect may also have an adverse impact on human health. In this work we offer a quantitative theory of roughness resistance and vibration that links these effects to a surface characterisation in terms of the International Roughness Index (IRI). We show that the roughness resistance and the Vibration Dose Value (or VDV, the usual vibration dosage metric) can be expressed in terms of elementary formulae. The roughness resistance depends only on the vertical stiffness of the bicycle and the roughness index. Surprisingly, other apparently relevant parameters, such as physiological characteristics of the bicycle rider and other features of the bicycle, do not enter. For roads of moderate roughness, roughness resistance is larger than rolling resistance. For very rough roads, roughness resistance is larger than aerodynamic drag. So only on roads of high quality (in most jurisdictions, accounting for less than 10~\% of the total) can roughness resistance be ignored. Roughness resistance can be mitigated by reducing the vertical stiffness of the bicycle. In common with other recent reports, we find that almost any cycling activity will breach public health guidelines relating to Vibration Dose Value.",2405.00019v1 2015-05-11,Pressure-induced semimetal to superconductor transition in a three-dimensional topological material ZrTe5,"As a new type of topological materials, ZrTe5 shows many exotic properties under extreme conditions. Utilizing resistance and ac magnetic susceptibility measurements under high pressure, while the resistance anomaly near 128 K is completely suppressed at 6.2 GPa, a fully superconducting transition emerges surprisingly. The superconducting transition temperature Tc increases with applied pressure, and reaches a maximum of 4.0 K at 14.6 GPa, followed by a slight drop but remaining almost constant value up to 68.5 GPa. At pressures above 21.2 GPa, a second superconducting phase with the maximum Tc of about 6.0 K appears and coexists with the original one to the maximum pressure studied in this work. In situ high-pressure synchrotron X-ray diffraction and Raman spectroscopy combined with theoretical calculations indicate the observed two-stage superconducting behavior is correlated to the structural phase transition from ambient Cmcm phase to high-pressure C2/m phase around 6 GPa, and to a mixture of two high-pressure phases of C2/m and P-1 above 20 GPa. The combination of structure, transport measurement and theoretical calculations enable a complete understanding of the emerging exotic properties in three-dimensional topological materials happened under extreme environments.",1505.02658v2 2015-08-05,Screening and transport in 2D semiconductor systems at low temperatures,"Low temperature carrier transport properties in two-dimensional (2D) semiconductor systems can be theoretically well-understood within a mean-field type RPA-Boltzmann theory as being limited by scattering from screened Coulomb disorder arising from random quenched charged impurities in the environment. In the current work, we derive a number of simple analytical formula, supported by realistic numerical calculations, for the relevant density, mobility, and temperature range where 2D transport should manifest strong intrinsic (i.e., arising purely from electronic effects and not from phonon scattering) metallic temperature dependence in different semiconductor materials arising entirely from the 2D screening properties, thus providing an explanation for why the strong temperature dependence of the 2D resistivity can only be observed in high-quality and low-disorder (i.e., high-mobility) 2D samples and also why some high-quality 2D materials (i.e., n-GaAs) manifest much weaker metallicity than other materials. We also discuss effects of interaction and disorder on the 2D screening properties in this context as well as compare 2D and 3D screening functions to comment why such a strong intrinsic temperature dependence arising from screening cannot occur in 3D metallic carrier transport. Experimentally verifiable predictions are made about the quantitative magnitude of the maximum possible low-temperature metallicity in 2D systems and the scaling behavior of the temperature scale controlling the quantum to classical crossover where the system reverses the sign of the temperature derivative of the 2D resistivity at high temperatures.",1508.01195v1 2007-07-04,Role of oxygen vacancies in Cr-doped SrTiO3 for resistance-change memory,"Transition-metal oxides exhibiting a bistable resistance state are attractive for non-volatile memory applications. The relevance of oxygen vacancies (VO) for the resistance-change memory was investigated with x-ray fluorescence, infrared microscopy, and x-ray absorption spectroscopy using Cr-doped SrTiO3 as example. We propose that the microscopic origin of resistance switching in this class of materials is due to an oxygen-vacancy drift occurring in close proximity to one of the electrodes.",0707.0563v1 2012-12-17,Measurement of specific contact resistivity using scanning voltage probes,"Specific contact resistivity measurements have conventionally been heavy in both fabrication and simulation/calculation in order to account for complicated geometries and other effects such as parasitic resistance. We propose a simpler geometry to deliver current, and the use of a scanning voltage probe to sense the potential variation along the sample surface, from which the specific contact resistivity can be straightforwardly deduced. We demonstrate an analytical example in the case where both materials are thin films. Experimental data with a scanning Kelvin probe measurement on graphene from the literature corroborates our model calculation.",1212.4182v2 2013-11-04,Surface resistivity of hydrogenated amorphous carbon films: Existence of intrinsic graphene on its surface,"Surface resistivity of hydrogenated amorphous carbon films was measured as a function of the applied electrical field. The measured dependence shows a sharp ambipolar peak near zero gate voltage. Furthermore, we found that in some samples sheet resistance at the peak is as low as 7.5 k{\Omega}/sq. This value is the same order of magnitude as the sheet resistance of a defect free graphene monolayer. Therefore a conclusion is made that an intrinsic graphene with dimensions of at least millimeters exist on the surface of amorphous carbon films. These results can open new perspectives not only for graphene applications, but also for better understanding of this unique material.",1311.0605v2 2014-06-17,High-Performance MoS2 Field-Effect Transistors Enabled by Chloride Doping: Record Low Contact Resistance (0.5 kohm*um) and Record High Drain Current (460 uA/um),"In this paper, we report a novel chemical doping technique to reduce the contact resistance (Rc) of transition metal dichalcogenides (TMDs) - eliminating two major roadblocks (namely, doping and high Rc) towards demonstration of high-performance TMDs field-effect transistors (FETs). By using 1,2 dichloroethane (DCE) as the doping reagent, we demonstrate an active n-type doping density > 2*1019 cm-3 in a few-layer MoS2 film. This enabled us to reduce the Rc value to a record low number of 0.5 kohm*um, which is ~10x lower than the control sample without doping. The corresponding specific contact resistivity (pc) is found to decrease by two orders of magnitude. With such low Rc, we demonstrate 100 nm channel length (Lch) MoS2 FET with a drain current (Ids) of 460 uA/um at Vds = 1.6 V, which is twice the best value reported so far on MoS2 FETs.",1406.4492v1 2015-04-14,Thermal boundary resistance at Si/Ge interfaces determined by approach-to-equilibrium molecular dynamics simulations,"The thermal boundary resistance of Si/Ge interfaces as been determined using approach-to-equilibrium molecular dynamics simulations. Assuming a reciprocal linear dependence of the thermal boundary resistance, a length-independent bulk thermal boundary resistance could be extracted from the calculation resulting in a value of 3.76x10$^{-9}$ m$^2$ K/W for a sharp Si/Ge interface and thermal transport from Si to Ge. Introducing an interface with finite thickness of 0.5 nm consisting of a SiGe alloy, the bulk thermal resistance slightly decreases compared to the sharp Si/Ge interface. Further growth of the boundary leads to an increase in the bulk thermal boundary resistance. When the heat flow is inverted (Ge to Si), the thermal boundary resistance is found to be higher. From the differences in the thermal boundary resistance for different heat flow direction, the rectification factor of the Si/Ge has been determined and is found to significantly decrease when the sharp interface is moderated by introduction of a SiGe alloy in the boundary layer.",1504.03613v1 2019-06-12,Kapitza resistance in basic chain models with isolated defects,"Kapitza thermal resistance is a common feature of material interfaces. It is defined as the ratio of the thermal drop at the interface to the heat flux flowing across the interface. One expects that this resistance will depend on the structure of the interface and on the temperature. We address the heat conduction in one-dimensional chain models with isotopic and/or coupling defects and explore the relationship between the interaction potentials and simulated properties of the Kapitza resistance. It is revealed that in linear models the Kapitza resistance is well-defined and size-independent (contrary to the bulk heat conduction coefficient), but depends on the parameters of thermostats used in the simulation. For $\beta$-FPU model one also encounters the dependence on the thermostats; in addition, the simulated boundary resistance strongly depends on the total system size. Finally, in the models characterized by convergent bulk heat conductivity (chain of rotators, Frenkel-Kontorova model) the boundary resistance is thermostat- and size-independent, as one expects. In linear chains, the Kapitza resistance is temperature-independent; thus, its temperature dependence allows one to judge on significance of the nonlinear interactions in the phonon scattering processes at the interface.",1906.05152v1 2022-09-22,Computational Design of Corrosion-resistant and Wear-resistant Titanium Alloys for Orthopedic Implants,"Titanium alloys are promising candidates for orthopedic implants due to their mechanical resilience and biocompatibility. Current titanium alloys in orthopedic implants still suffer from low wear and corrosion resistance. Here, we present a computational method for optimizing the composition of titanium alloys for enhanced corrosion and wear resistance without compromising on other aspects such as phase stability, biocompatibility, and strength. We use the cohesive energy, oxide formation energy, surface work function, and the elastic shear modulus of pure elements as proxy descriptors to guide us towards alloys with enhanced wear and corrosion resistance. For the best-selected candidates, we then use the CALPHAD approach, as implemented in the Thermo-Calc software, to calculate the phase diagram, yield strength, hardness, Pourbaix diagram, and the Pilling-Bedworth (PB) ratio. These calculations are used to assess the thermodynamic stability, biocompatibility, corrosion resistance, and wear resistance of the selected alloys. Additionally, we provide insights about the role of silicon on improving the corrosion and wear resistance of alloys.",2210.00845v1 2021-08-17,"Superconducting-like and magnetic transitions in oxygen-implanted diamond-like and amorphous carbon films, and in highly oriented pyrolytic graphite","In our previously published work, we have reported colossal magnetoresistance, Andreev oscillations, ferromagnetism, and granular superconductivity in oxygen-implanted carbon fibers, graphite foils, and highly oriented pyrolytic graphite. In this follow-up research, more results on these oxygen-implanted graphite samples are presented. We show results from transport measurements on oxygen-implanted diamond-like carbon thin coatings, amorphous carbon films, and highly oriented pyrolytic graphite. Significantly, a three-order magnitude drop in the electrical resistance of the oxygen-implanted diamond-like carbon films is observed at the 50 K temperature that we have previously reported for the transition to the superconducting state. Below 50 K, the films resistance oscillates between the high and low resistance states, less when the sample is under a transverse magnetic field. This metastability between the insulating and superconducting-like states possibly reflects the evolution of the amplitude for the superconducting order parameter also known as the longitudinal Higgs mode. Transitions to low resistance state and metastability are also observed for amorphous carbon films. Finally, the highly oriented pyrolytic graphite samples resistance have a thermally activated term that can be understood on the basis of the LAMH model applied to narrow SC channels in which thermal fluctuations can cause phase slips. We also find that in oxygen-implanted carbon materials, the electron charge and spin correlations do not compete and their interplay rather facilitates the emergence of high-temperature superconductivity, and thus, additional unexpected effects like Heisenberg spin waves and magneto-structural transitions are observed.",2108.07417v1 2019-11-20,Aspects of the Normal State Resistivity of Cuprate Superconductors,"Planar normal state resistivity data taken from three families of cuprate superconductors are compared with theoretical calculations from the recent extremely correlated Fermi liquid theory (ECFL). The two hole doped cuprate materials $LSCO$ and $BSLCO$ and the electron doped material $LCCO$ have yielded rich data sets at several densities $\delta$ and temperatures T, thereby enabling a systematic comparison with theory. The recent ECFL resistivity calculations for the highly correlated $t$-$t'$-$J$ model by us give the resistivity for a wide set of model parameters. After using X-ray diffraction and angle resolved photoemission data to fix parameters appearing in the theoretical resistivity, only one parameter, the magnitude of the hopping $t$, remains undetermined. For each data set, the slope of the experimental resistivity at a single temperature-density point is sufficient to determine $t$, and hence the resistivity on absolute scale at all remaining densities and temperatures. This procedure is shown to give a fair account of the entire data.",1911.09119v3 2005-10-20,Dependence of tunnel magnetoresistance in MgO based magnetic tunnel junctions on Ar pressure during MgO sputtering,"We investigated dependence of tunnel magnetoresistance effect in CoFeB/MgO/CoFeB magnetic tunnel junctions on Ar pressure during MgO-barrier sputtering. Sputter deposition of MgO-barrier at high Ar pressure of 10 mTorr resulted in smooth surface and highly (001) oriented MgO. Using this MgO as a tunnel barrier, tunnel magnetoresistance (TMR) ratio as high as 355% at room temperature (578% at 5K) was realized after annealing at 325 C or higher, which appears to be related to a highly (001) oriented CoFeB texture promoted by the smooth and highly oriented MgO. Electron-beam lithography defined deep-submicron MTJs having a low-resistivity Au underlayer with the high-pressure deposited MgO showed high TMR ratio at low resistance-area product (RA) below 10 ohm-um^2 as 27% at RA = 0.8 ohm-um^2, 77% at RA = 1.1 ohm-um^2, 130% at RA = 1.7 ohm-um^2, and 165% at RA = 2.9 ohm-um^2.",0510531v1 2014-09-23,Fabrication of Flexible Super Capacitor Using Laser Lightscribe Technique,"Super capacitors are promising energy storage devices due to their capability of delivering high peak current and storing high amount of energy in a short time with very low internal power loss. We fabricated the graphene or graphite oxide super-capacitor using laser Lightscribe technique. We prepared graphite oxide by modified hummers method and used PET film as a flexible substrate on which graphite oxide (GO) was coated. Using Lightscribe drive and software, the super-capacitor configuration was patterned on the GO coated PET film. During the writing process, the laser converts GO into graphene. We characterized the fabricated flexible super-capacitor which exhibits high resistance of 20KOhm with applied voltage of 10V and further increase of voltage (20V) decreases the resistance to 8KOhm. We also analyzed the frequency response of the capacitor using impedance measurement which shows high frequency response and estimated capacitance is 120nF. We optimized the patterns by running the Lightscribe repeatedly on the GO coated PET substrate.",1409.6396v1 2019-09-20,Extraordinary high room-temperature carrier mobility in graphene-WSe$_2$ heterostructures,"High carrier mobilities play a fundamental role for high-frequency electronics, integrated optoelectronics as well as for sensor and spintronic applications, where device performance is directly linked to the magnitude of the carrier mobility. Van der Waals heterostructures formed by graphene and hexagonal boron nitride (hBN) already outperform all known materials in terms of room temperature mobility. Here, we show that the mobility of today's best graphene/hBN devices can be surpassed by more than a factor of three by heterostructures formed by tungsten diselenide (WSe$_2$), graphene and hBN, which can have mobilities as high as 350,000 cm$^2$/(Vs) at room temperature, and resistivities as low as 15 Ohm. The resistivity of these devices shows a much weaker temperature dependence than the one of graphene on any other known substrate. The origin of this behaviour points to modified acoustic phonon bands in graphene and questions our understanding of electron-phonon scattering in van der Waals heterostructures.",1909.09523v1 2015-06-29,High quality monolayer graphene synthesized by resistive heating cold wall chemical vapour deposition,"Emerging flexible and wearable technologies such as healthcare electronics and energy-harvest devices could be transformed by the unique properties of graphene. The vision for a graphene-driven industrial revolution is motivating intensive research on the synthesis of (1) high quality and (2) low cost graphene. Hot-wall chemical vapour deposition (CVD) is one of the most competitive growth methods, but its long processing times are incompatible with production lines. Here we demonstrate the growth of high quality monolayer graphene using a technique that is 100 times faster than standard hot-wall CVD, resulting in 99% reduction in production costs. A thorough complementary study of Raman spectroscopy, atomic force microscopy, scanning electron microscopy and electrical magneto-transport measurements shows that our cold wall CVD-grown graphene is of comparable quality to that of natural graphene. Finally, we demonstrate the first transparent and flexible graphene capacitive touch-sensor that could enable the development of artificial skin for robots.",1506.08569v1 2015-09-29,A Nonlinear HP-Type Complementary Resistive Switch,"Resistive Switching (RS) is the change in resistance of a dielectric under the influence of an external current or electric field. This change is non-volatile, and the basis of both the memristor and resistive random access memory. In the latter, high integration densities favor the anti-serial combination of two RS-elements to a single cell, termed the complementary resistive switch (CRS). Motivated by the irregular shape of the filament protruding into the device, we suggest a nonlinearity in the resistance-interpolation function, and thereby expand the original HP-memristor. We numerically simulate and analytically solve this model. Further, the nonlinearity allows for its application to the CRS.",1509.08885v1 2003-08-14,Resistivity Ratio of Niobium Superconducting Cavities,"Resistivity measurements have been made on Nb cavities, as well as on Pb and Cu, at 296, 77, and 4.2 K by means of a contactless induced-current method. For superconductors, a constant magnetic field drives the material normal below the transition temperature. These measurements provide a simple means for initial material evaluation as well as a direct means of monitoring the effects of material parameters (purity, heat treatment, gas incorporation, etc.) on the electron mean free path. Approximate determinations of Hc, Hc1, and Hc2 can also be derived from these measurements. Normal-state thermal conductivity and the Ginzburg-Landau parameter kappa are calculated from the resistivity measurements.",0308266v1 2014-01-09,Rapid Embedded Wire Heating via Resistive Guiding of Laser-Generated Fast Electrons as a Hydrodynamic Driver,"Resistively guiding laser-generated fast electron beams in targets consisting of a resistive wire embedded in lower $Z$ material should allow one to rapidly heat the wire to over 100eV over a substantial distance without strongly heating the surrounding material. On the multi-ps timescale this can drive hydrodynamic motion in the surrounding material. Thus ultra-intense laser solid interactions have the potential as a controlled driver of radiation hydrodynamics in solid density material. In this paper we assess the laser and target parameters needed to achieve such rapid and controlled heating of the embedded wire.",1401.1998v1 2002-07-19,Spin Injection: Interface Resistance in Fe/Semiconductor Junctions Calculated from First Principles,"We calculate the current spin polarisation and the interface resistance of Fe/GaAs and Fe/ZnSe (001) spin injection junctions from first principles, including also the possibility of a Schottky barrier. From our results of interface resistance we estimate the barrier thickness needed for efficient spin injection if the process is non-ballistic.",0207492v1 2007-08-01,Resistance noise in Bi_2Sr_2CaCu_2O$_{8+δ}$,"The resistance noise in a Bi_2Sr_2CaCu_2O$_{8+\delta}$ thin film is found to increase strongly in the underdoped regime. While the increase of the raw resistance noise with decreasing temperature appears to roughly track the previously reported pseudogap temperature for this material, standard noise analysis rather suggests that the additional noise contribution is driven by the proximity of the superconductor-insulator transition.",0708.0117v1 2010-06-14,A conjecture of Biggs concerning the resistance of a distance-regular graph,"Previously, Biggs has conjectured that the resistance between any two points on a distance-regular graph of valency greater than 2 is bounded by twice the resistance between adjacent points. We prove this conjecture, give the sharp constant for the inequality, and display the graphs for which the conjecture most nearly fails. Some necessary background material is included, as well as some consequences.",1006.2687v1 2019-06-13,"Comment on arXiv:1807.08572, ""Coexistence of Diamagnetism and Vanishingly Small Electrical Resistance at Ambient Temperature and Pressure in Nanostructures""","A recent preprint arXiv:1807.08572 reported the observation of a transition in Ag/Au nanoparticle composites near room temperature and at ambient pressure, to a vanishingly small four-probe resistance, which was tentatively identified as a percolating superconducting transition. In this brief comment, I point out that a vanishing four-probe resistance may also emerge in non-superconducting systems near conductance percolation threshold.",1906.05742v1 2017-08-18,A New Method for Characterizing Bulk and Surface Conductivities of Three-Dimensional Topological Insulators: Inverted Resistance Measurements,"We introduce a new resistance measurement method that is useful in characterizing materials with both surface and bulk conduction, such as three-dimensional topological insulators. The transport geometry for this new resistance measurement configuration consists of one current lead as a closed loop that fully encloses the other current lead on the surface, and two voltage leads that are both placed outside the loop. We show that in the limit where the transport is dominated by the surface conductivity of the material, the four-terminal resistance measured from such a transport geometry is proportional to $\sigma_b/\sigma_s^2$, where $\sigma_b$ and $\sigma_s$ are the bulk and surface conductivities of the material, respectively. We call this new type of measurement \textit{inverted resistance measurement}, as the resistance scales inversely with the bulk resistivity. We discuss possible implementations of this new method by performing numerical calculations on different geometries and introduce strategies to extract the bulk and surface conductivities. We also demonstrate inverted resistance measurements on SmB$_6$, a topological Kondo insulator, using both single-sided and coaxially-aligned double-sided Corbino disk transport geometries. Using this new method, we are able to measure the bulk conductivity, even at low temperatures, where the bulk conduction is much smaller than the surface conduction in this material.",1708.05762v2 2007-11-02,Effects of carbon nanotubes on grain boundary sliding in zirconia polycrystals,"Mechanical properties of zirconia polycrystals decrease drastically at high temperature due to thermally activated grain boundary (GB) sliding, leading to plastic or even super-plastic deformation. As GB sliding is a source of energy dissipation in the material, mechanical loss measurements are well suited to study such a mechanism. They reveal, in general, a mechanical loss peak, which evolves into an exponential increase at higher temperature. When intergranular glassy films or/and amorphous pockets are presented in polycrystalline ceramics, the mechanical loss is globally higher and so is the creep rate. Here we show that introducing carbon nanotubes in zirconia, in particular, reduces drastically GB sliding and consequently the mechanical loss at high temperature. The nanotubes were observed at the grain boundaries by high-resolution transmission electron microscopy and were related to the reduction of superplasic flow through the boundaries, which should improve the material creep resistance.",0711.0381v1 2010-01-25,"High-pressure synthesis, crystal and electronic structures of a new scandium tungstate, Sc0.67WO4","Negative thermal expansion (NTE) materials possess a low-density, open structure which can respond to high pressure conditions, leading to new compounds and/or different physical properties. Here we report that one such NTE material -- white, insulating, orthorhombic Sc2W3O12 -- transforms into a black compound when treated at 4 GPa and 1400 oC. The high pressure phase, Sc0.67WO4, crystallizes in a defect-rich wolframite-type structure, a dense, monoclinic structure (space group P2/c) containing 1-D chains of edge-sharing WO6 octahedra. The chemical bonding of Sc0.67WO4 vis-a-vis the ambient pressure Sc2W3O12 phase can be understood on the basis of the Sc defect structure. Magnetic susceptibility, resistivity, thermoelectric power and IR spectroscopic measurements reveal that Sc0.67WO4 is a paramagnet whose conductivity is that of a metal in the presence of weak localization and electron-electron interactions. Oxygen vacancies are suggested as a potential mechanism for generating the carriers in this defective wolframite material.",1001.4561v1 2016-10-18,Low Temperature Thermoelectric Properties of Co- and Cr- doped CuAgSe,"High mobility phonon-glass semimetal $CuAgSe$ has shown promise in recent years as a potential low-temperature thermoelectric material. It exhibits reasonably strong thermoelectric performance as well as an extremely high carrier mobility, both of which are enhanced when the material is doped with Ni at the Cu sites. The exact mechanism by which these enhancements result; however, is unclear. In order to further investigate the effects of chemical substitution on the material's thermoelectric properties, we have prepared and performed various measurements on $CuAgSe$ samples doped with Co and Cr according to the following compositional formulas: $Cu_{1-x}Co_{x}AgSe$ $(x=0.02, 0.05, 0.10)$ and $Cu_{1-x}Cr_{x}AgSe$ $(x=0.02, 0.05)$. Measurements of temperature and magnetic field dependent thermal conductivity, electrical resistivity, and Seebeck coefficient will be discussed. Our results reveal a remarkable sensitivity of $CuAgSe$'s thermoelectric properties to chemical doping in general as well as a particular sensitivity to specific dopants. This demonstrated tunability of $CuAgSe$'s various properties furthers the case that high mobility phonon glass-semimetals are strong candidates for potential low temperature thermoelectric applications.",1610.05634v1 2018-03-14,Ultra High Molecular Weight Polyethylene: optical features at millimeter wavelengths,"The next generation of experiments for the measurement of the Cosmic Microwave Background (CMB) requires more and more the use of advanced materials, with specific physical and structural properties. An example is the material used for receiver's cryostat windows and internal lenses. The large throughput of current CMB experiments requires a large diameter (of the order of 0.5m) of these parts, resulting in heavy structural and optical requirements on the material to be used. Ultra High Molecular Weight (UHMW) polyethylene (PE) features high resistance to traction and good transmissivity in the frequency range of interest. In this paper, we discuss the possibility of using UHMW PE for windows and lenses in experiments working at millimeter wavelengths, by measuring its optical properties: emissivity, transmission and refraction index. Our measurements show that the material is well suited to this purpose.",1803.05228v1 2019-08-02,Machine-learning-assisted thin-film growth: Bayesian optimization in molecular beam epitaxy of SrRuO3 thin films,"Materials informatics exploiting machine learning techniques, e.g., Bayesian optimization (BO), has the potential to offer high-throughput optimization of thin-film growth conditions through incremental updates of machine learning models in accordance with newly measured data. Here, we demonstrated BO-based molecular beam epitaxy (MBE) of SrRuO3, one of the most-intensively studied materials in the research field of oxide electronics, mainly owing to its unique nature as a ferromagnetic metal. To simplify the intricate search space of entangled growth conditions, we ran the BO for a single condition while keeping the other conditions fixed. As a result, high-crystalline-quality SrRuO3 film exhibiting a high residual resistivity ratio (RRR) of over 50 as well as strong perpendicular magnetic anisotropy was developed in only 24 MBE growth runs in which the Ru flux rate, growth temperature, and O3-nozzle-to-substrate distance were optimized. Our BO-based search method provides an efficient experimental design that is not as dependent on the experience and skills of individual researchers, and it reduces experimental time and cost, which will accelerate materials research.",1908.00739v1 2002-04-08,Pressure Effect on the Superconducting and Magnetic Transitions of the Superconducting Ferromagnet RuSr2GdCu2O8,"The superconducting ferromagnet RuSr2GdCu2O8 was investigated at high pressure. The intra-grain superconducting transition temperature, Tc, is resolved in ac-susceptibility as well as resistivity measurements. It is shown that the pressure shift of Tc is much smaller than that of other high-Tc compounds in a similar doping state. In contrast, the ferromagnetic transition temperature, Tm, increases with pressure at a relative rate that is about twice as large as that of Tc. The high-pressure data indicate a possible competition of the ferromagnetic and superconducting states in RuSr2GdCu2O8.",0204185v1 2004-09-23,Superconducting and Normal State Properties of Heavily Hole-Doped Diamond,"We report measurements of the specific heat, Hall effect, upper critical field and resistivity on bulk, B-doped diamond prepared by reacting amorphous B and graphite under high-pressure/high-temperature conditions. These experiments establish unambiguous evidence for bulk superconductivity and provide a consistent set of materials parameters that favor a conventional, weak coupling electron-phonon interpretation of the superconducting mechanism at high hole doping.",0409624v1 2000-04-10,Systematic evolution of the magnetotransport properties of Bi_{2}Sr_{2-x}La_{x}CuO_{6} in a wide doping range,"Recently we have succeeded in growing a series of high-quality Bi_{2}Sr_{2-x}La_{x}CuO_{6} crystals in a wide range of carrier concentrations. The data of \rho_{ab}(T) and R_H(T) of those crystals show behaviors that are considered to be ""canonical"" to the cuprates. The optimum zero-resistance T_c has been raised to as high as 38 K, which is almost equal to the optimum T_c of La_{2-x}Sr_{x}CuO_{4}.",0004134v1 2005-07-20,Superconductivity in Polycrystalline Diamond Thin Films,"Superconductivity was discovered in heavily boron-doped diamond thin films deposited by the microwave plasma assisted chemical vapor deposition (MPCVD) method. Advantages of the MPCVD deposited diamond are the controllability of boron concentration in a wide range, and a high boron concentration, especially in (111) oriented films, compared to that of the high-pressure high-temperature method. The superconducting transition temperatures are determined to be 8.7K for Tc onset and 5.0K for zero resistance by transport measurements. And the upper critical field is estimated to be around 7T.",0507476v2 2006-11-15,"Silicon detectors: damage, modelling and expected long-time behaviour in physics experiments at ultra high energy","In this contribution, the structural modifications of the material and the degradation of devices is modelled and compared with experimental data for more resistivities, temperatures, crystal orientations and oxygen concentrations, considering the existence of the new primary fourfold coordinated defect, besides the vacancy and the interstitial. Some estimations of the behaviour of detectors in concrete environments at the next generations of high energy physics experiments as LHC, SLHC, VLHC, or ULHC are done.",0611142v1 2008-01-07,High pressure-high temperature phase diagram of ammonia,"The high pressure(P)-high temperature(T) phase diagram of solid ammonia has been investigated using diamond anvil cell and resistive heating techniques. The III-IV transition line has been determined up to 20 GPa and 500 K both on compression and decompression paths. No discontinuity is observed at the expected location for the III-IV-V triple point. The melting line has been determined by visual observations of the fluid-solid equilibrium up to 9 GPa and 900 K. The experimental data is well fitted by a Simon-Glatzel equation in the covered P-T range. These transition lines and their extrapolations are compared with reported calculations.",0801.0913v1 2008-07-16,High-Temperature Superconductivity in Eu0.5K0.5Fe2As2,"Subsequent to our recent report of SDW type transition at 190 K and antiferromagnetic order below 20 K in EuFe2As2, we have studied the effect of K-doping on the SDW transition at high temperature and AF order at low temperature. 50% K doping suppresses the SDW transition and in turn gives rise to high-temperature superconductivity below T_c = 32 K, as observed in the electrical resistivity, AC susceptibility as well as magnetization. A well defined anomaly in the specific heat provides additional evidence for bulk superconductivity.",0807.2530v2 2017-09-08,Room temperature ferromagnetism in transparent and conducting Mn-doped $SnO_{2}$ thin films,"The magnetization as a function of magnetic field showed hysteretic behavior at room temperature. According to the temperature dependence of the magnetization, the Curie temperature $(T_{C})$ is higher than 350 K. Ferromagnetic Mn-doped tin oxide thin films exhibited low electrical resistivity and high optical transmittance in the visible region (400-800 nm). The coexistence of ferromagnetism, high visible transparency and high electrical conductivity in the Mn-doped $SnO_{2}$ films is expected to be a desirable trait for spintronics devices.",1709.05930v1 2020-11-18,The CLICTD Monolithic CMOS Sensor,"CLICTD is a monolithic silicon pixel sensor fabricated in a modified 180 nm CMOS imaging process with a small collection electrode design and a high-resistivity epitaxial layer. It features an innovative sub-pixel segmentation scheme and is optimised for fast charge collection and high spatial resolution. The sensor was developed to target the requirements for the tracking detector of the proposed future Compact Linear Collider (CLIC). Most notably, a temporal resolution of a few nanoseconds and a spatial resolution below 7 microns are demanded. In this contribution, the sensor performance measured in beam tests is presented with emphasis on recent studies using assemblies with different thicknesses (down to 50 microns to minimize the material budget) and inclined particle tracks.",2011.09389v1 2023-11-28,A Brief Review and Perspective on the Functional Biodegradable Films for Food Packaging,"High-performance, environmentally-friendly biodegradable packaging as substitutes for conventional plastics becomes severe demand to nowadays economy and society. As an aliphatic aromatic copolyester PBAT is recognized as the preferred alternative to traditional plastics. However, the relatively high cost and weak properties obstacles the widespread adoption of PBAT. Modification pertaining to improve the properties, lower the cost, and include the functional additives of PBAT is a continuous effort to meet the needs of food accessibility, antibacterial properties, oxygen resistance, high mechanical strength, stable size, low moisture absorption, and various gas permeability for commercial competitiveness.",2311.16932v1 2023-05-18,Indium-Tin-Oxide for High-performance Electro-optic Modulation,"Advances in opto-electronics are often led by discovery and development of materials featuring unique properties. Recently the material class of transparent conductive oxides (TCO) has attracted attention for active photonic devices on-chip. In particular Indium Tin Oxide (ITO) is found to have refractive index changes on the order of unity. This property makes it possible to achieve electro-optic modulation of sub-wavelength device scales, when thin ITO films are interfaced with optical light confinement techniques such as found in plasmonics; optical modes are compressed to nanometer scale to create strong light-matter-interactions. Here we review efforts towards utilizing this novel material for high-performance and ultra-compact modulation. While high performance metrics are achieved experimentally, there are open questions pertaining the permittivity modulation mechanism of ITO. Furthermore, we show that a footprint-saving waveguide inline cavity can enhance obtainable extinction-ratio to insertion-loss ratios by about one order of magnitude over non-cavity based version. Moreover, we offer a speed analysis that shows that the device is resistance limited, but not capacitance or drift-carrier limited. Interestingly, two bias options exist for ITO and we find that a side-connection enables devices that should in principle enable several hundred of GHz fast devices, using our routinely achievable ITO film resistivities. Finally, we offer a brief discuss about footprint savings of compact ITO modulators showing a 3-orders of magnitude smaller footprint over Silicon photonic MZI-based modulators.",2305.10639v1 2024-03-14,"Magnetotransport properties in van-der-Waals \textit{\textbf{R}}Te$_{3}$ (\textit{\textbf{R}} = La, Ce, Tb)","Rare-earth tritellurides are van-der-Waals antiferromagnets which have been attracting attention as materials not only with high mobility, but also with various states such as superconductivity under high pressure, incommensurate charge-density-wave (CDW) phase, and multiple antiferromagnetic phases. In this work, we performed longitudinal resistivity and Hall resistivity measurements simultaneously in exfoliated $R$Te$_{3}$ ($R$ =La, Ce, Tb) thin film devices, in order to investigate the influence of magnetic ordering on transport properties in van-der-Waals magnetic materials. We have obtained carrier mobility and concentration using a two-band model, and have observed an increase in carrier mobility in the antiferromagnets CeTe$_{3}$ and TbTe$_{3}$ due to the magnetic transition. Especially in CeTe$_{3}$, the carrier concentration has changed drastically below the magnetic transition temperature, suggesting the interaction between the CDW and antiferromagnetic phases. In addition, the analysis of the Shubnikov-de Haas oscillations in CeTe$_{3}$ supports the possibility of Fermi surface modulation by magnetic ordering. This research will pave the way not only for spintronic devices that take advantage of high mobility, but also for the study of the correlation between CDW and magnetism states in low-dimensional materials.",2403.09250v2 2016-02-19,Magnetic effects in sulfur-decorated graphene,"The interaction between two different materials can present novel phenomena that are quite different from the physical properties observed when each material stands alone. Strong electronic correlations, such as magnetism and superconductivity, can be produced as the result of enhanced Coulomb interactions between electrons. Two-dimensional materials are powerful candidates to search for the novel phenomena because of the easiness of arranging them and modifying their properties accordingly. In this work, we report magnetic effects of graphene, a prototypical non-magnetic two-dimensional semi-metal, in the proximity with sulfur, a diamagnetic insulator. In contrast to the well-defined metallic behaviour of clean graphene, an energy gap develops at the Fermi energy for the graphene/sulfur compound with decreasing temperature. This is accompanied by a steep increase of the resistance, a sign change of the slope in the magneto-resistance between high and low fields, and magnetic hysteresis. A possible origin of the observed electronic and magnetic responses is discussed in terms of the onset of low-temperature magnetic ordering. These results provide intriguing insights on the search for novel quantum phases in graphene-based compounds.",1602.06214v2 2020-09-27,Non-equilibrium Effects in Dissipative Strongly Correlated Systems,"Novel physics arises when strongly correlated system is driven out of equilibrium by external fields. Dramatic changes in physical properties, such as conductivity, are empirically observed in strongly correlated materials under high electric field. In particular, electric-field driven metal-insulator transitions are well-known as the resistive switching effect in a variety of materials, such as VO$_2$, V$_2$O$_3$ and other transition metal oxides. To satisfactorily explain both the phenomenology and its underlying mechanism, it is required to model microscopically the out-of-equilibrium dissipative lattice system of interacting electrons. In this thesis, we developed a systematic method of modeling non-equilibrium steady states for dissipative lattice systems by means of Non-equilibrium Green's function and Dynamical Mean Field Theory. We firstly establish a ""minimum model"" to formulate the strong-field transport in non-interacting dissipative electron lattice. This model is exactly soluble and convenient for discussing energy dissipation and steady-state properties. The formalism is then combined with Dynamical Mean Field Theory to provide a systematic framework describing the nonequilibrium steady-state of correlated materials. We use the formalism to study the strong-field transport properties of correlated materials, Mott insulators and Dirac electrons in graphene. We concentrate on the microscopic description of resistive switching. Of particular interest is the filament formation during the dynamical phase transition, which has been interpreted as a result of the delicate interplay between dissipation and Mott physics. We will also examine $IV$ characteristics and particularly the current saturation of Dirac electrons in graphene. The arXiv version has been updated with minor modifications and corrections.",2009.12865v1 2020-09-28,A hybrid optoelectronic Mott insulator,"The coupling of electronic degrees of freedom in materials to create hybridized functionalities is a holy grail of modern condensed matter physics that may produce novel mechanisms of control. Correlated electron systems often exhibit coupled degrees of freedom with a high degree of tunability which sometimes lead to hybridized functionalities based on external stimuli. However, the mechanisms of tunability and the sensitivity to external stimuli are determined by intrinsic material properties which are not always controllable. A Mott metal-insulator transition, which is technologically attractive due to the large changes in resistance, can be tuned by doping, strain, electric fields, and orbital occupancy but cannot be, in and of itself, controlled externally with light. Here we present a new approach to produce hybridized functionalities using a properly engineered photoconductor/strongly-correlated hybrid heterostructure, showing control of the Metal-to-Insulator transition (MIT) using optical means. This approach combines a photoconductor, which does not exhibit an MIT, with a strongly correlated oxide, which is not photoconducting. Due to the close proximity between the two materials, the heterostructure exhibits large volatile and nonvolatile, photoinduced resistivity changes and substantial photoinduced shifts in the MIT transition temperatures. This approach can potentially be extended to other judiciously chosen combinations of strongly correlated materials with systems which exhibit optically, electrically or magnetically controllable behavior.",2009.13606v1 2020-01-02,Thermal Conductivity Measurements in Nanosheets via Bolometric Effect,"Thermal conductivity measurement techniques for materials with nanoscale dimensions require fabrication of very complicated devices or their applicability is limited to a class of materials. Discovery of new methods with high thermal sensitivity are required for the widespread use of thermal conductivity measurements in characterizing materials properties. We propose and demonstrate a simple non-destructive method with superior thermal sensitivity to measure the in-plane thermal conductivity of nanosheets and nanowires using the bolometric effect. The method utilizes laser beam heating to create a temperature gradient, as small as a fraction of a Kelvin, over the suspended section of the nanomaterial with electrical contacts. Local temperature rise due to the laser irradiation alters the electrical resistance of the device, which can be measured precisely. This resistance change is then used to extract the temperature profile along the nanomaterial using thermal conductivity as a fitting parameter. We measured the thermal conductivity of V2O3 nanosheets to validate the applicability of the method and found an excellent agreement with the literature. Further, we measured the thermal conductivity of metallic 2H-TaS2 for the first time and performed ab initio calculations to support our measurements. Finally, we discussed the applicability of the method on semiconducting nanosheets and performed measurements on WS2 and MoS2 thin flakes.",2001.00368v1 2020-11-01,Bipolar Magnetic Semiconducting Behavior in VNbRuAl: A New Spintronic Material for Spin Filters,"We report the theoretical prediction of a new class of spintronic materials, namely bipolar magnetic semiconductor (BMS), which is also supported by our experimental data. BMS acquires a unique band structure with unequal band gaps for spin up and down channels, and thus are useful for tunable spin transport based applications such as spin filters. The valence band (VB) and conduction band (CB) in BMS approach the Fermi level through opposite spin channels, and hence facilitate to achieve reversible spin polarization which are controllable via applied gate voltage. We report the quaternary Heusler alloy VNbRuAl to exactly possess the band structure of BMS. The alloy is found to crystallize in LiMgPdSn prototype structure (space group $F\bar{4}3m$) with B$2$ disorder and lattice parameter 6.15 \AA . The resistivity and Hall measurements show a two channel semiconducting behavior and a quasi linear dependence of negative magneto resistance (MR) indicating the possible semiconducting nature. Interestingly, VNbRuAl also shows a fully compensated ferrimagnetic (FCF) behavior with vanishing net magnetization (m$_s$$\sim$ $10^{-3}$ $\mu_B/f.u.$) and significantly high ordering temperature ($> 900$ K). Unlike conventional FCF, vanishing moment in this case appears to be the result of a combination of long range antiferromagnetic (AFM) ordering and the inherent B2 disorder of the crystal. This study opens up the possibility of finding a class of materials for AFM spintronics, with great significance both from fundamental and applied fronts.",2011.00533v1 2021-10-26,Wet Scandium Etching for hard mask formation on a silicon substrate,"Nowadays, microelectronics and nanoelectronics require the search for new materials, including masks for creating structures. Today, the intermediate hard mask strategy is one of the key issues in achieving a good balance between lithography and etching at the microelectronic fabrication. One of the interesting challenges in microelectronics and photovoltaics is the creation of interspacing, vertically oriented silicon arrays on Si substrate for semiconductor devices with multi-function. The fabrication of such structures is still a serious technological problem and requires searching for new approaches and materials. In this work, we propose using scandium as a new hard mask material over silicon due to its high resistance to plasma chemical etching and low sputtering coefficient. We have shown that a wet etching of the scandium layer with a thickness of several nanometers can be used to obtain pattern structures with a resolution of up to 4 microns, which is a good result for the wet etching approach. Scandium metal was found to be an excellent resistant mask over silicon under the selected plasma etching conditions. Therefore, a scandium hard mask can open up new possibilities for the formation of different microscale topographical patterns.",2110.13639v3 2007-01-03,Two-dimensional Vortices in Superconductors,"Superconductors have two key characteristics. They expel magnetic field and they conduct electrical current with zero resistance. However, both properties are compromised in high magnetic fields which can penetrate the material and create a mixed state of quantized vortices. The vortices move in response to an electrical current dissipating energy which destroys the zero resistance state\cite{And64}. One of the central problems for applications of high temperature superconductivity is the stabilization of vortices to ensure zero electrical resistance. We find that vortices in the anisotropic superconductor Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+\delta}$ (Bi-2212) have a phase transition from a liquid state, which is inherently unstable, to a two-dimensional vortex solid. We show that at high field the transition temperature is independent of magnetic field, as was predicted theoretically for the melting of an ideal two-dimensional vortex lattice\cite{Fis80,Gla91}. Our results indicate that the stable solid phase can be reached at any field as may be necessary for applications involving superconducting magnets\cite{Has04,Sca04,COHMAG}. The vortex solid is disordered, as suggested by previous studies at lower fields\cite{Lee93,Cub93}. But its evolution with increasing magnetic field displays unexpected threshold behavior that needs further investigation.",0701059v1 2007-11-01,Point-contact search for antiferromagnetic giant magnetoresistance,"We report the first measurements of effects of large current densities on current-perpendicular-to-plane magnetoresistance (MR) of magnetic multilayers containing two antiferromagnetic layers separated by a non-magnetic layer. These measurements were intended to search for a recently predicted antiferromagnetic giant magnetoresistance (AGMR) similar to GMR seen in multilayers containing two ferromagnetic layers separated by a non-magnetic layer. We report on MR measurements for current injected from point contacts into sandwiches containing different combinations of layers of F = CoFe and AFM = FeMn. In addition to: AFM/N/AFM, F/AFM/N/AFM, and F/AFM/N/AFM/F structures, initial results led us to examine also AFM/F/N/AFM, F/AFM, and single F- and AFM-layer structures. At low currents, no MR was observed in any samples, and no MR was observed at any current densities in samples containing only AFMs. Together, these results indicate that no AGMR is present in these samples. In samples containing F-layers, high current densities sometimes produced a small positive MR - largest resistance at high fields. For a given contact resistance, this MR was usually larger for thicker F-layers, and for a given current, it was usually larger for larger contact resistances (smaller contacts). We tentatively attribute this positive MR to suppression at high currents of spin accumulation induced around and within the F-layers.",0711.0059v3 2008-06-18,Linear-T resistivity and change in Fermi surface at the pseudogap critical point of a high-Tc superconductor,"A fundamental question of high-temperature superconductors is the nature of the pseudogap phase which lies between the Mott insulator at zero doping and the Fermi liquid at high doping p. Here we report on the behaviour of charge carriers near the zero-temperature onset of that phase, namely at the critical doping p* where the pseudogap temperature T* goes to zero, accessed by investigating a material in which superconductivity can be fully suppressed by a steady magnetic field. Just below p*, the normal-state resistivity and Hall coefficient of La1.6-xNd0.4SrxCuO4 are found to rise simultaneously as the temperature drops below T*, revealing a change in the Fermi surface with a large associated drop in conductivity. At p*, the resistivity shows a linear temperature dependence as T goes to zero, a typical signature of a quantum critical point. These findings impose new constraints on the mechanisms responsible for inelastic scattering and Fermi surface transformation in theories of the pseudogap phase.",0806.2881v2 2016-06-07,Spin-Orbit Interaction and Kondo Scattering at the PrAlO$_3$/SrTiO$_3$ Interface: Effects of Oxygen Content,"We report the effect of oxygen pressure during growth ($P_{O_{2}}$) on the electronic and magnetic properties of PrAlO$_3$ films grown on $\rm TiO_{2}$-terminated SrTiO$_3$ substrates. Resistivity measurements show an increase in the sheet resistance as $P_{O_{2}}$ is increased. The temperature dependence of the sheet resistance at low temperatures is consistent with Kondo theory for $P_{O_{2}} \ge 10^{-5}$ torr. Hall effect data exhibit a complex temperature dependence that suggests a compensated carrier density. We observe behavior consistent with two different types of carriers at interfaces grown at $P_{O_{2}} \ge 10^{-4}$ torr. For these interfaces, we measured a moderate positive magnetoresistance (MR) due to a strong spin-orbit (SO) interaction at low magnetic fields that evolves into a larger negative MR at high fields. Positive high MR values are associated with samples where a fraction of carriers are derived from oxygen vacancies. Analysis of the MR data permitted the extraction of the SO interaction critical field ( e.g. $ H_{SO}=$1.25 T for $P_{O_{2}}=10^{-5}$ torr). The weak anti-localization effect due to a strong SO interaction becomes smaller for higher $P_{O_{2}}$ grown samples, where MR values are dominated by the Kondo effect, particularly at high magnetic fields.",1606.02308v1 2016-07-20,Magnetotransport properties of the type II Weyl semimetal candidate Ta3S2,"We have investigated the magnetoresistance (MR) and Hall resistivity properties of the single crystals of tantalum sulfide, Ta3S2, which was recently predicted to be a new type II Weyl semimetal. Large MR (up to ~8000% at 2 K and 16 T), field-induced metal-insulator-like transition and nonlinear Hall resistivity are observed at low temperatures. The large MR shows a strong dependence on the field orientation, leading to a giant anisotropic magnetoresistance (AMR) effect. For the field applied along the b-axis (B//b), MR exhibits quadratic field dependence at low fields and tends towards saturation at high fields; while for B//a, MR presents quadratic field dependence at low fields and becomes linear at high fields without any trend towards saturation. The analysis of the Hall resistivity data indicates the coexistence of a large number of electrons with low mobility and a small number of holes with high mobility. Shubnikov-de Haas (SdH) oscillation analysis reveals three fundamental frequencies originated from the three-dimensional (3D) Fermi surface (FS) pockets. We find that the semi-classical multiband model is sufficient to account for the experimentally observed MR in Ta3S2.",1607.05798v2 2017-10-25,Device model for pixelless infrared image up-converters based on polycrystalline graphene heterostructures,"We develop a device model for pixelless converters of far/mid-infrared radiation (FIR/MIR) images into near-infrared/visible (NIR/VIR) images. These converters use polycrystalline graphene layers (PGLs) immersed in the van der Waals (vdW) materials integrated with light emitting diode (LED). The PGL serves as an element of the PGL infrared photodetector (PGLIP) sensitive to the incoming FIR/MIR due to the interband absorption. The spatially non-uniform photocurrent generated in the PGLIP repeats (mimics) the non-uniform distribution (image) created by the incident FIR/MIR. The injection of the nonuniform photocurrent into the LED active layer results in the nonuniform NIR/VIR image reproducing the FIR/MIR image. The PGL and the entire layer structure are not deliberately partitioned into pixels. We analyze the characteristics of such pixelless PGLIP-LED up-converters and show that their image contrast transfer function and the up-conversion efficiency depend on the PGL lateral resistivity. The up-converter exhibits high photoconductive gain and conversion efficiency when the lateral resistivity is sufficiently high. Several teams have successfully demonstrated the large area PGLs with the resistivities varying in a wide range. Such layers can be used in the pixelless PGLIP-LED image up-converters. The PGLIP-LED image up-converters can substantially surpass the image up-converters based on the quantum-well infrared photodetector (QWIP) integrated with the LED. These advantages are due to the use of the interband FIR/NIR absorption and a high photoconductive gain in the GLIPs.",1710.09060v1 2018-06-18,Electroluminescence on-off ratio control of n-i-n GaAs/AlGaAs-based resonant tunneling structures,"We explore the nature of the electroluminescence (EL) emission of purely n-doped GaAs/AlGaAs resonant tunneling diodes (RTDs) and the EL evolution with voltage. A singular feature of such a device is unveiled when the electrical output current changes from high to low and the EL on-off ratio is enhanced by 2 orders of magnitude compared to the current on-off ratio. By combining the EL and current properties, we are able to identify two independent impact ionization channels associated with the coherent resonant tunneling current and the incoherent valley current. We also perform the same investigation with an associated series resistance, which induces a bistable electrical output in the system. By simulating a resistance variation for the current-voltage and the EL, we are able to tune the EL on-off ratio by up to 6 orders of magnitude. We further observe that the EL on and off states can be either direct or inverted compared to the tunneling current on and off states. This electroluminescence, combined with the unique RTD properties such as the negative differential resistance (NDR) and high frequency operation, enables the development of high speed functional opto-electronic devices and optical switches.",1806.06757v1 2012-01-19,Magnetic Field Effects on Transport Properties of PtSn4,"The anisotropic physical properties of single crystals of orthorhombic PtSn4 are reported for magnetic fields up to 140 kOe, applied parallel and perpendicular to the crystallographic b-axis. The magnetic susceptibility has an approximately temperature independent behavior and reveals an anisotropy between ac-plane and b-axis. Clear de Haas-van Alphen oscillations in fields as low as 5 kOe and at temperatures as high as 30 K were detected in magnetization isotherms. The thermoelectric power and resistivity of PtSn4 show the strong temperature and magnetic field dependencies. A change of the thermoelectric power at H = 140 kOe is observed as high as ~ 50 mu-V/K. Single crystals of PtSn4 exhibit very large transverse magnetoresistance of ~ 5x10^5% for the ac-plane and of ~ 1.4x10^5% for the b-axis resistivity at 1.8 K and 140 kOe, as well as pronounced Shubnikov-de Haas oscillations. The magnetoresistance of PtSn4 appears to obey Kohler's rule in the temperature and field range measured. The Hall resistivity shows a linear temperature dependence at high temperatures followed by a sign reversal around 25 K which is consistent with thermoelectric power measurements. The observed quantum oscillations and band structure calculations indicate that PtSn4 has three dimensional Fermi surfaces.",1201.4091v1 2020-10-23,"Air-stable, earth-abundant molten chlorides and corrosion-resistant containment for chemically-robust, high-temperature thermal energy storage for concentrated solar power","A dramatic reduction in man-made CO2 emissions could be achieved if the cost of electricity generated from concentrated solar power (CSP) plants could become competitive with fossil-fuel-derived electricity. The solar heat-to-electricity conversion efficiency of CSP plants may be significantly increased (and the associated electricity cost decreased) by operating CSP turbines with inlet temperatures >750 C instead of <550 C, and by using thermal energy storage (TES) at >750 C to allow for rapidly dispatchable and/or continuous electricity production. Unfortunately, earth-abundant MgCl2-KCl-based liquids currently being considered as low-cost media for large-scale, high-temperature TES are susceptible to oxidation in air, with associated undesired changes in liquid composition and enhanced corrosion of metal alloys in pipes and tanks containing such liquids. In this paper, alternative high-temperature, earth-abundant molten chlorides that are stable in air are identified via thermodynamic calculations. The oxidation resistance, and corrosion-resistant containment, of such molten chlorides at 750 C are then demonstrated. Such chemically-robust, low-cost TES media and effective containment provide critical advances towards the higher-temperature operation of, and lower-cost electricity generation from, CSP plants.",2010.12476v1 2023-03-03,Anomalous Random Telegraphy Signal in Suspended Graphene with Oxygen Adsorption,"Graphene is a promising material for sensing applications because of its large specific surface area and low noise. In many applications, graphene will inevitably be in contact with oxygen since it is the second most abundant gas in the atmosphere. Therefore, it is of interest to understand how this gas affects the sensor properties. In this work, the effect of oxygen on the low-frequency noise of suspended graphene is demonstrated. Devices with suspended graphene nanoribbons with a width (W) and length (L) of 200 nm were fabricated. The resistance as a function of time was measured in a vacuum and pure oxygen atmosphere through an ac lock-in method. After signal processing with wavelet denoising and analysis, it is demonstrated that oxygen causes random telegraphy signal (RTS) in the millisecond scale, with an average dwell time of 2.9 milliseconds in the high-resistance state, and 2 milliseconds in the low-resistance state. It is also shown that this RTS occurs only at some periods, which indicates that, upon adsorption, the molecules take some time until they find the most energetically favorable adsorption state. Also, a slow-down in the RTS time constants is observed, which infers that less active sites are available as time goes on because of oxygen adsorption. Therefore, it is very important to consider these effects to guarantee high sensitivity and high durability for graphene-based sensors that will be exposed to oxygen during their lifetime.",2303.01649v2 2007-09-12,Characterization of Thermal Interface Materials to Support Thermal Simulation,"In this paper new characterization equipment for thermal interface materials is presented. Thermal management of electronic products relies on the effec-tive dissipation of heat. This can be achieved by the optimization of the system design with the help of simulation methods. The precision of these models relies also on the used material data. For the determi-nation of this data an experimental set-up for a static measurement is presented, which evaluates thermal conductivity and interface resistance of thermal inter-face materials (e.g. adhesive, solder, pads, or pastes). A qualitative structure-property correlation is pro-posed taking into account particle size, filler content and void formation at the interface based on high resolution FIB imaging. The paper gives an overview over the set-up and the measurement technique and discusses experimental and simulation results.",0709.1849v1 2016-02-29,A Solid-State Dielectric Elastomer Switch for Soft Logic,"In this paper we describe a stretchable solid-state electronic switching material that operates at high voltage potentials, as well as a switch material benchmarking technique that utilizes a modular dielectric elastomer (artificial muscle) ring oscillator. The solid-state switching material was integrated into our oscillator, which self-started after 16s and performed 5 oscillations at a frequency of 1.05Hz with 3.25kV DC input. Our materials-by-design approach for the nickel filled polydimethysiloxane (Ni-PDMS) based switch has resulted in significant improvements over previous carbon-grease based switches in four key areas, namely sharpness of switching behavior upon applied stretch, magnitude of electrical resistance change, ease of manufacture, and rate of production. Switch lifetime was demonstrated to be in the range of tens to hundreds of cycles with the current process. An interesting and potentially useful strain-based switching hysteresis behavior is also presented.",1602.08988v1 2019-03-15,An efficient phase-field model for fatigue fracture in ductile materials,"Fatigue fracture in ductile materials, e. g. metals, is caused by cyclic plasticity. Especially regarding the high numbers of load cycles, plastic material models resolving the full loading path are computationally very demanding. Herein, a model with particularly small computational effort is presented. It provides a macroscopic, phenomenological description of fatigue fracture by combining the phase-field method for brittle fracture with a classic durability concept. A local lifetime variable is obtained, which degrades the fracture resistance progressively. By deriving the stress-strain path from cyclic material characteristics, only one increment per load cycle is needed at maximum. The model allows to describe fatigue crack initiation, propagation and residual fracture and can reproduce Paris behaviour.",1903.06465v3 2021-10-21,Structures and physical properties of V-based kagome metals CsV$_{6}$Sb$_{6}$ and CsV$_{8}$Sb$_{12}$,"We report two new members of V-based kagome metals CsV$_{6}$Sb$_{6}$ and CsV$_{8}$Sb$_{12}$. The most striking structural feature of CsV$_{6}$Sb$_{6}$ is the V kagome bilayers. For CsV$_{8}$Sb$_{12}$, there is an intergrowth of two-dimensional V kagome layers and one-dimensional V chains and the latter lead to the orthorhombic symmetry of this material. Further measurements indicate that these two materials exhibit metallic and Pauli paramagnetic behaviors. More importantly, different from CsV$_{3}$Sb$_{5}$, the charge density wave state and superconductivity do not emerge in CsV$_{6}$Sb$_{6}$ and CsV$_{8}$Sb$_{12}$ when temperature is above 2 K. Small magnetoresistance with saturation behavior and linear field dependence of Hall resistivity at high field and low temperature suggest that the carriers in both materials should be uncompensated with much different concentrations. The discovery of these two new V-based kagome metals sheds light on the exploration of correlated topological materials based on kagome lattice.",2110.11452v2 2022-05-17,The Highly Disordered Zintl Phase Ca$_{10}$GdCdSb$_9$ -- New Example of a p-type Semiconductor with Remarkable Thermoelectric Properties,"Ca$_{10}$GdCdSb$_9$ is a new Zintl phase with a large unit cell volume (~2500 {\AA}3) and a very complex, disordered structure, which can drive the realization of ultralow thermal conductivity in this material. The measured Seebeck coefficient, $\alpha$, for single-crystalline Ca$_{10}$GdCdSb$_9$ approaches 350 $\mu$V/K at 600 K. The experimentally determined electrical resistivity of Ca$_{10}$GdCdSb$_9$ is very low, leading to a remarkably high-power factor PF of 23.2 $\mu$W/cm.K$^2$ at 460 K. The extraordinary PF value in this material, higher than those of the currently known state-of-the-art materials within the same temperature range, suggests that the Ca$_{10}$RECdSb$_9$ material system (RE = rare earth metal) could serve as a viable playground to harnessing new efficient thermoelectric generators.",2205.08559v1 2022-10-12,Experimental data management platform for data-driven investigation of combinatorial alloy thin films,"Experimental materials data are heterogeneous and include a variety of metadata for processing and characterization conditions, making the implementation of data-driven approaches for developing novel materials difficult. In this paper, we introduce the Thin-Film Alloy Database (TFADB), a materials data management platform, designed for combinatorially investigated thin-film alloys through various experimental tools. Using TFADB, researchers can readily upload, edit, and retrieve multidimensional experimental alloy data, such as composition, thickness, X-ray Diffraction, electrical resistivity, nanoindentation, and image data. Furthermore, composition-dependent properties from the database can easily be managed in a format adequate to be preprocessed for machine learning analyses. High flexibility of the software allows management of new types of materials data that can be potentially acquired from new combinatorial experiments.",2210.06027v1 2022-10-18,Reaction-diffusion pathways for a programmable nanoscale texture of diamond-SiC composite,"The diamond-SiC composite has a low density and the highest possible speed of sound among existing materials except for the diamond. The composite is synthesized by a complex exothermic chemical reaction between diamond powder and liquid Si. This makes it an ideal material for protection against impact loading. Experiments show that a system of patterns is formed at the diamond-SiC interface. Modeling of reaction-diffusion processes of composite synthesis proves a formation of ceramic materials with a regular (periodic) interconnected microstructure in a given system. Composite material with interconnected structures at the interface has very high mechanical properties and resistance to impact since its fractioning is intercrystallite.",2210.10021v1 2023-11-02,Machine Learning Design of Perovskite Catalytic Properties,"Discovering new materials that efficiently catalyze the oxygen reduction and evolution reactions is critical for facilitating the widespread adoption of solid oxide fuel cell and electrolyzer (SOFC/SOEC) technologies. Here, we develop machine learning (ML) models to predict perovskite catalytic properties critical for SOFC/SOEC applications, including oxygen surface exchange, oxygen diffusivity, and area specific resistance (ASR). The models are based on trivial-to-calculate elemental features and are more accurate and dramatically faster than the best models based on ab initio-derived features, potentially eliminating the need for ab initio calculations in descriptor-based screening. Our model of ASR enables temperature-dependent predictions, has well calibrated uncertainty estimates and online accessibility. Use of temporal cross-validation reveals our model to be effective at discovering new promising materials prior to their initial discovery, demonstrating our model can make meaningful predictions. Using the SHapley Additive ExPlanations (SHAP) approach, we provide detailed discussion of different approaches of model featurization for ML property prediction. Finally, we use our model to screen more than 19 million perovskites to develop a list of promising cheap, earth-abundant, stable, and high performing materials, and find some top materials contain mixtures of less-explored elements (e.g., K, Bi, Y, Ni, Cu) worth exploring in more detail.",2311.01401v1 2024-01-22,Order induces toughness in anisotropic colloidal crystal composites,"Spatial ordering of matter elicits exotic properties sometimes absent from a material's constituents. A few highly mineralised natural materials achieve high toughness through delocalised damage, whereas synthetic particulate composites must trade toughness for mineral content. We test whether ordering the mineral phase in particulate composites through the formation of macroscopic colloidal crystals can trigger the same damage resistance found in natural materials. Our macroscopic silica rod based anisotropic colloidal crystal composites are processed fully at room temperature and pressure, reach volume fraction of mineral higher than 80%, and aided by a ductile interface, unveil plastic strain reaching 10% through the collective movement of rods and damage delocalisation over millimetres. These composites demonstrate key design rules to break free from conventionally accepted structural materials properties trade-off.",2401.11727v1 2016-10-24,Probing Intrinsic Material Conductivity in Two-Terminal Devices: A Resistance-Difference Method,"It is generally impossible to separately measure the resistance of the functional component (i.e., the intrinsic device materials) and the parasitic component (i.e., terminals, interfaces and serial loads) in a two-terminal device. Yet such knowledge is important for understanding device physics and designing device systems. Here, we consider a case where an electric current, temperature, or magnetic field causes a small but identical relative conductivity change of the device materials. We find an exact solution to this relative change by a simple resistance-data analysis of similarly configured two-terminal devices. The solution is obtainable even if the change is quite small, say, less than 0.1%. In special cases of small relative changes in parasitic resistance, the absolute parasitic resistance is also obtainable. Our method is especially useful for studying the switching and transport characteristics of the emergent non-volatile resistance memory.",1610.07666v2 2018-03-22,Status and update of the RaDIATE Collaboration R&D Program,"The Radiation Damage In Accelerator Target Environments (RaDIATE) collaboration was founded in 2012 and currently consists of over 50 participants and 11 institutions globally. Due to the increasing power of future proton accelerator sources in target facilities, there is a critical need to further understand the physical and thermo-mechanical radiation response of target facility materials. Thus, the primary objective of the RaDIATE collaboration is to draw on existing expertise in the nuclear materials and accelerator targets fields to generate new and useful materials data for application within the accelerator and fission/fusion communities. Current research activities of the collaboration include post irradiation examination (PIE) of decommissioned components from existing beamlines such as the NuMI beryllium beam window and graphite NT-02 target material. PIE of these components includes advanced microstructural analyses (SEM/TEM, EBSD, EDS) and micro-mechanics technique such as nano-indentation, to help characterize any microstructural radiation damage incurred during operation. New irradiation campaigns of various candidate materials at both low and high energy beam facilities are also being pursued. Beryllium helium implantation studies at the University of Surrey as well as high energy proton irradiation of various materials at Brookhaven National Laboratory's BLIP facility have been initiated. The program also extends to beam-induced thermal shock experiments using high intensity beam pulses at CERN's HiRadMat facility, followed by advanced PIE activities to evaluate thermal shock resistance of the materials. Preliminary results from ongoing research activities, as well as the future plans of the RaDIATE collaboration R&D program will be discussed.",1803.08563v1 2021-12-22,Self-repairing high entropy oxides,"All biological organisms, from plants to living creatures, can heal minor wounds and damage. The realization of a similar self-healing capacity in inorganic materials has been a design target for many decades. This would represent a breakthrough in materials engineering, enabling many novel technological applications, since such materials would be able to resist damage caused by electromagnetic irradiation and/or mechanical impact. Here we demonstrate that a high-entropy oxide is intrinsically capable of undergoing an autonomous self-repairing process. Transmission electron microscopy revealed that the spinel structure of (AlCoCrCu0.5FeNi)3O4 can regrow and repair itself at the atomic level when damaged. Density functional theory calculations reveal that the extra enthalpy stored in the high entropy material during fabrication can be released to effectively heal macroscopic defects by regrowing into a partially ordered state. This extraordinary self-repairing phenomenon makes this new material highly desirable as a coating, enabling structures used in harsh environments to better withstand damage, such as cosmic irradiation in space, nuclear irradiation in nuclear power facilities, or tribological damage. Most importantly, our results set the general design principles for the synthesis of self-repairing materials.",2112.11747v1 2004-01-23,"Crystal growth and anisotropic transport properties of high-Tc superconductors Bi2Sr2Can-1CunO2n+4+d (n = 2, 3)","Large high-quality single crystals of Bi2Sr2Can-1CunO2n+4+d (n = 2, 3) were successfully grown using an improved traveling solvent floating zone (TSFZ) method, which features a slow growth rate and steep temperature gradient along the melting zone. By measuring anisotropic resistivities and susceptibilities of Bi2Sr2CaCu2O8+d, the characteristic pseudogap temperature T* was studied as a function of doping. The T* suggest that the pseudogap is not simply a precursor of high-Tc superconductivity, but that the pseudogap and the superconducting gap compete with each other. The anisotropic resistivities of Bi2Sr2Ca2Cu3O10+d were also measured, revealing that the Tc remains fixed in the overdoped region while anisotropy decreases continuously. This anomalous behavior will be discussed in terms of the inequivalent hole doping, which occurs between two inequivalent CuO2 planes in the triple-layer system.",0401448v3 2010-04-28,Conductivity states changes in plasticized PVC films near breakdown threshold voltages values,"The near threshold ""soft breakdown"" measurements of PVC films conductivity are investigated. In a wide range of external electric field strength for various rather thick (>20 mkm) PVC films the resistance shows strong nonlinearity and seems to enter high conductive state close to the breakdown threshold. For our ""thick"" films boundary conditions electrode surface specifics should not be so important as in thin polymer films experiments. Both fast, instant mechanisms of nonlinearity, and effects of accumulation and delay responce were observed. The phenomena corresponding to reversible transitions in a state with rather high conductivity, seems to be similar to ones registered earlier in thin layers of some broad-bandgap polymers. In a range of relatively low field intensity, far from a threshold breakdown, as a result of reversible switches between normal and high resistivity states a polymer film in a standard measuring cell formed a relaxation generator giving a loud enough sound signal with frequency increasing with the increase of external field.",1004.4972v1 2010-12-27,Superconductivity and Magnetic Properties of high-quality single crystals of $A_{x}$Fe$_2$Se$_2$ ($A$ = K and Cs),"We successfully grew the high-quality single crystals of $A_{x}$Fe$_2$Se$_2$ ($A$ = K and Cs) by self-flux method. Sharp superconducting transition was observed for both types of crystals. The crystals show the onset superconducting transition temperatures ($T_{\rm c}$) of 31 K and 30 K for K- and Cs-compounds, respectively, with nearly 100% shielding fraction. The crystals show quite high resistivity in the normal state of more than 160 m$\Omega$ cm and 1300 m$\Omega$ cm maximum resistivity for $K_{0.86}Fe_2Se_{1.82}$ and $Cs_{0.86}Fe_{1.66}Se_{2}$ single crystals, respectively. Much larger upper critical field $H_{\rm c2}$ is inferred from low-temperature iso-magnetic-field magnetoresistance in these crystals than in FeSe. The anisotropy $H^{ab}_{\rm c2}$(0)/$H^{c}_{\rm c2}$(0) is around 3 for both of the two materials. Anisotropic peculiar magnetic behavior in normal state has been found for $Cs_{0.86}Fe_{1.66}Se_{2}$",1012.5552v1 2015-09-15,Epitaxial graphene quantum dots for high-performance THz bolometers,"Light absorption in graphene causes a large change in electron temperature, due to low electronic heat capacity and weak electron phonon coupling [1-3], making it very attractive as a hot-electron bolometer material. Unfortunately, the weak variation of electrical resistance with temperature has substantially limited the responsivity of graphene bolometers. Here we show that quantum dots of epitaxial graphene on SiC exhibit an extraordinarily high variation of resistance with temperature due to quantum confinement, higher than 430 Mohm/K at 2.5 K, leading to responsivities for absorbed THz power above 10^10 V/W. This is five orders of magnitude higher than other types of graphene hot electron bolometers. The high responsivity combined with an extremely low noise-equivalent power, about 0.2 fW/Hz^0.5 at 2.5K, place the performance of graphene quantum dot bolometers well above commercial cooled bolometers. Additionally, these quantum dot bolometers have the potential for superior performance for operation above 77K.",1509.04646v1 2016-11-15,Linear magnetoresistance in a quasi-free two dimensional electron gas in an ultra-high mobility GaAs quantum well,"We report a magnetotransport study of an ultra-high mobility ($\bar{\mu}\approx 25\times 10^6$\,cm$^2$\,V$^{-1}$\,s$^{-1}$) $n$-type GaAs quantum well up to 33 T. A strong linear magnetoresistance (LMR) of the order of 10$^5$ % is observed in a wide temperature range between 0.3 K and 60 K. The simplicity of our material system with a single sub-band occupation and free electron dispersion rules out most complicated mechanisms that could give rise to the observed LMR. At low temperature, quantum oscillations are superimposed onto the LMR. Both, the featureless LMR at high $T$ and the quantum oscillations at low $T$ follow the empirical resistance rule which states that the longitudinal conductance is directly related to the derivative of the transversal (Hall) conductance multiplied by the magnetic field and a constant factor $\alpha$ that remains unchanged over the entire temperature range. Only at low temperatures, small deviations from this resistance rule are observed beyond $\nu=1$ that likely originate from a different transport mechanism for the composite fermions.",1611.04857v1 2017-02-24,Elemental Analysis of Glass and Bakelite Electrodes Using PIXE Facility,"The evolution of particle detectors dates back to the discovery of X-rays and radioactivity in 1890s. In detector history, the Resistive Plate Chambers (RPCs) are introduced in early 1980s. An RPC is a gaseous detector made up of two parallel electrodes having high resistivity like that of glass and bakelite. Currently several high energy physics experiments are using RPC-based detector system due to robustness and simplicity of construction. In each and every experiment, RPCs have to run continuously for several years. So, it demands an in-depth characterization of the electrode materials. In the present study, an elemental analysis of locally available glass and bakelite samples is done using PIXE facility available at Panjab University Cyclotron, Chandigarh. PIXE measurements are done using 2.7 MeV proton beam incident on the electrode sample target. The constituent elements present in these electrode samples are reported.",1702.08480v3 2014-08-12,Collapse of CuO Double Chains and Suppression of Superconductivity in High-Pressure Phase of YBa$_2$Cu$_4$O$_8$,"The crystal structure and electrical resistivity of YBa$_2$Cu$_4$O$_8$ (Y124) were studied under high pressure up to 18 GPa using diamond-anvil cells, respectively, in order to clarify its conduction mechanism. Y124 causes the first-order phase-transition into the orthorhombic Immm at pressure around 11 GPa. The high-pressure phase (HPP) also shows the superconductivity, while the manner of temperature dependence of electrical resistance and the pressure dependence of transition temperature, Tc, drastically change above 11 GPa. The CuO$_2$ plane persists in HPP but the CuO double chains collapse with the phase transition and transform into three-dimensional Cu-O network, resulting in the renewal of conduction system.",1408.2613v1 2019-02-11,Improved oxidation resistance of high emissivity coatings on fibrous ceramic for reusable space system,"To develop high emissivity coatings on fibrous ceramic substrates with improved thermal resistance for reusable space systems, WSi2-MoSi2-Si-SiB6-borosilicate glass coatings were prepared on fibrous ZrO2 by slurry dipping and subsequent high temperature rapid sintering. A coating with 50 wt% WSi2 and 50 wt% MoSi2 presents optimal thermal stability with only 10.06 mg/cm2 mass loss and 4.0 % emissivity decrease in the wavelength regime of 1.27 to 1.73 microns after 50 h oxidation at 1773 K. The advantages of double phase metal silicide coatings combining WSi2 and MoSi2 include improved thermal compatibility with the substrate and an enhanced glass mediated self healing ability.",1902.03943v2 2018-08-16,Investigating Unipolar Switching in Niobium Oxide Resistive Switches: Correlating Quantized Conductance and Mechanism,"Memory devices based on resistive switching (RS) have not been fully realised due to lack of understanding of the underlying switching mechanisms. Nature of ion transport responsible for switching and growth of conducting filament in transition metal oxide based RS devices is still in debate. Here, we investigated the mechanism in Niobium oxide based RS devices, which shows unipolar switching with high ON/OFF ratio, good endurance cycles and high retention times. We controlled the boundary conditions between low-conductance insulating and a high-conductance metallic state where conducting filament (CF) can form atomic point contact and exhibit quantized conductance behaviour. Based on the statistics generated from quantized steps data, we demonstrated that the CF is growing atom by atom with the applied voltage sweeps. We also observed stable quantized states, which can be utilized in multistate switching.",1808.05600v1 2019-12-19,A high-throughput structural and electrochemical study of metallic glass formation in Ni-Ti-Al,"Based on a set of machine learning predictions of glass formation in the Ni-Ti-Al system, we have undertaken a high-throughput experimental study of that system. We utilized rapid synthesis followed by high-throughput structural and electrochemical characterization. Using this dual-modality approach, we are able to better classify the amorphous portion of the library, which we found to be the portion with a full-width-half-maximum (FWHM) of 0.42 A$^{-1}$ for the first sharp x-ray diffraction peak. We demonstrate that the FWHM and corrosion resistance are correlated but that, while chemistry still plays a role, a large FWHM is necessary for the best corrosion resistance.",1912.09330v1 2011-04-22,High purity semi-insulating 4H-SiC epitaxial layers by Defect-Competition Epitaxy,"Thick, high-purity semi-insulating (SI)homoepitaxial layers on Si-face 4H-SiC weregrownsystematically, with resistivity \geq 109{\Omega}-cmby maintaining high C/Si ratios 1.3-15 during growth.Comparison of secondary ion mass spectra betweenlow-dopedepilayers grown at C/Si ratio<1.3andSI-epilayers grown at C/Si ratio>1.3 showed little difference in residual impurity concentrations. A reconciliation of impurity concentration with measured resistivity indicated a compensating trap concentration of ~1015cm-3present only in the SI-epilayers. High- resolution photo induced transient spectroscopy (HRPITS) identified themas Si-vacancy related deep centers, with no detectable EH6/7 and Z1/2levels. Recombination lifetimes ~5ns suggest application in fast-switching power devices.",1104.4509v1 2020-05-22,Sharp negative differential resistance from vibrational mode softening in molecular junctions,"We unravel the critical role of vibrational mode softening in single-molecule electronic devices at high bias. Our theoretical analysis is carried out with a minimal model for molecular junctions, with mode softening arising due to quadratic electron-vibration couplings, and by developing a mean-field approach. We discover that the negative sign of the quadratic electron-vibration coupling coefficient can realize at high voltage a sharp negative differential resistance (NDR) effect with a large peak-to-valley ratio. Calculated current-voltage characteristics, obtained based on ab initio parameters for a nitro-substituted oligo(phenylene ethynylene) junction, agree very well with measurements. Our results establish that vibrational mode softening is a crucial effect at high voltage, underlying NDR, a substantial diode effect, and the breakdown of current-carrying molecular junctions.",2005.11365v1 2023-02-28,ZrNb(CO) RF superconducting thin film with high critical temperature in the theoretical limit,"Superconducting radio-frequency (SRF) resonators are critical components for particle accelerator applications, such as free-electron lasers, and for emerging technologies in quantum computing. Developing advanced materials and their deposition processes to produce RF superconductors that yield nanoohms surface resistances is a key metric for the wider adoption of SRF technology. Here we report ZrNb(CO) RF superconducting films with high critical temperatures (Tc) achieved for the first time under ambient pressure. The attainment of a Tc near the theoretical limit for this material without applied pressure is promising for its use in practical applications. A range of Tc, likely arising from Zr doping variation, may allow a tunable superconducting coherence length that lowers the sensitivity to material defects when an ultra-low surface resistance is required. Our ZrNb(CO) films are synthesized using a low-temperature (100 - 200 C) electrochemical recipe combined with thermal annealing. The phase transformation as a function of annealing temperature and time is optimized by the evaporated Zr-Nb diffusion couples. Through phase control, we avoid hexagonal Zr phases that are equilibrium-stable but degrade Tc. X-ray and electron diffraction combined with photoelectron spectroscopy reveal a system containing cubic ZrNb mixed with rocksalt NbC and low-dielectric-loss ZrO2. We demonstrate proof-of-concept RF performance of ZrNb(CO) on an SRF sample test system. BCS resistance trends lower than reference Nb, while quench fields occur at approximately 35 mT. Our results demonstrate the potential of ZrNb(CO) thin films for particle accelerator and other SRF applications.",2302.14410v2 2020-01-07,First principles evaluation of fcc ruthenium for use in advanced interconnects,"As the semiconductor industry turns to alternate conductors to replace Cu for future interconnect nodes, much attention as been focused on evaluating the electrical performance of Ru. The typical hexagonal close-packed (hcp) phase has been extensively studied, but relatively little attention has been paid to the face-centered cubic (fcc) phase, which has been shown to nucleate in confined structures and may be present in tight-pitch interconnects. Using \emph{ab initio} techniques, we benchmark the performance of fcc Ru. We find that the phonon-limited bulk resistivity of the fcc Ru is less than half of that of hcp Ru, a feature we trace back to the stronger electron-phonon coupling elements that are geometrically inherited from the modified Fermi surface shape of the fcc crystal. Despite this benefit of the fcc phase, high grain boundary scattering results in increased resistivity compared to Cu-based interconnects with similar average grain size. We find, however, that the line resistance of fcc Ru is lower than that of Cu below 21 nm line width due to the conductor volume lost to adhesion and wetting liners. In addition to studying bulk transport properties, we evaluate the performance of adhesion liners for fcc Ru. We find that it is energetically more favorable for fcc Ru to bind directly to silicon dioxide than through conventional adhesion liners such as TaN and TiN. In the case that a thin liner is necessary for the Ru deposition technique, we find that the vertical resistance penalty of a liner for fcc Ru can be up to eight times lower than that calculated for conventional liners used for Cu interconnects. Our calculations, therefore, suggest that the formation of the fcc phase of Ru may be a beneficial for advanced, low-resistance interconnects.",2001.02216v3 2021-12-12,Electric-field-driven resistive transition in multiferroic SrCo$_2$Fe$_{16}$O$_{27}$/Sr$_3$Co$_2$Fe$_{24}$O$_{41}$composite,"We report observation of electric-field-driven resistive transition at a characteristic threshold field $E_{th}(T)$ across a temperature range 10-200 K in an off-stoichiometric composite of (~80 vol%) W- and (~20 vol%) Z-type hexaferrites. The dielectric constant $\epsilon$ and the relaxation time constant $\tau$ too exhibit anomalous jump at $E_{th}(T)$. The $E_{th}(T)$, the extent of jump in resistivity ($\Delta\rho$), and the hysteresis associated with the jump [$\Delta E_{th}(T)$] are found to decrease systematically with the increase in temperature ($T$). Several temperature-driven phase transitions have also been noticed in low and high resistive states (LRS and HRS). The temperature-driven conduction turns out to be governed by activated hopping of small polarons at all the phases with electric ($E$) and magnetic ($H$) field dependent activation energy $U(E,H)$. Interestingly, as the temperature is raised, the $E$-driven conduction at a fixed temperature evolves from $\textit{Ohmic}$ to $\textit{non-Ohmic}$ across 10-200 K and within 110-200 K, $\rho$ follows three-dimensional variable range hopping (3D-VRH) with stretched exponential $\sim$ $exp[(E_0/E)^4]$ or power law $\sim$ $(E_0/E)^m$ ($m$ varies within $\sim$0.6-0.7 and $\sim$0.6-0.8 at LRS and HRS, respectively) dependence depending on the localization length ($\zeta_E$) to diffusion length ($d_E$) ratio associated with $E$-driven conduction. The $\rho(E,T)$ follows universal scaling only at LRS within 10-110 K but not at higher temperature or at HRS. The entire set of observations has been discussed within the framework of structural evolution of the point-defect (cation vacancies or oxygen excess) network. This comprehensive map of esoteric $\rho-E-T-H$ and $\epsilon-E-T-H$ patterns provides insights on defect driven effects in a composite useful for tuning both the resistive transition and multiferroicity.",2112.06246v1 2023-02-20,Observation of near room temperature thin film superconductivity of atmospherically stable Ag-Au mesoscopic thin film,"An environmentally stable mesoscopic thin film of Au of certain thickness has been deposited thermally on top of a Ag+ implanted oxide substrate to develop a close to room temperature superconductor. This thin film has been deposited in two different stages. Initially, a sol-gel derived ion conducting metal oxide (ICMO) thin film has been deposited by spin coating. Afterward, Ag+ has been introduced inside ICMO thin film by a chemical method. Following this, a thin layer of Au has been deposited on top of that Ag ion-implanted oxide via thermal evaporation. The temperature dependent resistivity (R-T) has been studied by four probe method. During high-to-low temperature sweep, around 240 K this thin film sample shows a sudden drop of resistance from 0.7 Ohm to 0.1 micro-Ohm. This 6-7 orders drop of resistance has been observed instantly within <0.1 K temperature variation of the sample. This transition temperature (TC) has been shifted toward the higher temperature by 5-6 degrees when temperature has been increased from low to the higher side. During 2nd and 3rd temperature cycling, both these transitions have been shifted by ~10 K towards room temperature w.r.t the earlier. However, after three successive temperature cycles, TC becomes stable and transitions occur close to 0 oC repeatedly. At the low resistance phase, current level has been varied from +100 mA to -100 mA which shows a random fluctuation of voltage drop within 10 nV range, indicating resistance under such circumstance is too low to measure by Delta mode electrical measurement (0.1 micro-Ohm). Besides, transition temperature reduces to lower temperature by 4 K, after applying 1 tesla magnetic field perpendicular to the thin film. Few YouTube video links of temperature dependent electrical characterization of such a thin film is given next to the acknowledgement section.",2302.09974v3 2023-10-11,Absence of topological Hall effect in Fe$_x$Rh$_{100-x}$ epitaxial films: revisiting their phase diagram,"A series of Fe$_x$Rh$_{100-x}$ ($30 \leq x \leq 57$) films were epitaxially grown using magnetron sputtering, and were systematically studied by magnetization-, electrical resistivity-, and Hall resistivity measurements. After optimizing the growth conditions, phase-pure Fe$_{x}$Rh$_{100-x}$ films were obtained, and their magnetic phase diagram was revisited. The ferromagnetic (FM) to antiferromagnetic (AFM) transition is limited at narrow Fe-contents with $48 \leq x \leq 54$ in the bulk Fe$_x$Rh$_{100-x}$ alloys. By contrast, the FM-AFM transition in the Fe$_x$Rh$_{100-x}$ films is extended to cover a much wider $x$ range between 33 % and 53 %, whose critical temperature slightly decreases as increasing the Fe-content. The resistivity jump and magnetization drop at the FM-AFM transition are much more significant in the Fe$_x$Rh$_{100-x}$ films with $\sim$50 % Fe-content than in the Fe-deficient films, the latter have a large amount of paramagnetic phase. The magnetoresistivity (MR) is rather weak and positive in the AFM state, while it becomes negative when the FM phase shows up, and a giant MR appears in the mixed FM- and AFM states. The Hall resistivity is dominated by the ordinary Hall effect in the AFM state, while in the mixed state or high-temperature FM state, the anomalous Hall effect takes over. The absence of topological Hall resistivity in Fe$_{x}$Rh$_{100-x}$ films with various Fe-contents implies that the previously observed topological Hall effect is most likely extrinsic. We propose that the anomalous Hall effect caused by the FM iron moments at the interfaces nicely explains the hump-like anomaly in the Hall resistivity. Our systematic investigations may offer valuable insights into the spintronics based on iron-rhodium alloys.",2310.07140v1 2022-06-22,Thermoelectric properties of high-entropy rare-earth cobaltates,"High-entropy concept introduced with a promising paradigm to obtain exotic physical properties has motivated us to explore the thermoelectric properties of Sr-substituted high-entropy rare-earth cobaltates i.e., (LaNdPrSmEu)$_{1-x}$Sr$_x$CoO3 (0 \leq x \leq 0.10). The structural analysis of the samples synthesized using the standard solid-state route, confirms the orthorhombic structure with the Pbnm space group. The Seebeck coefficient and electrical resistivity decrease with rising Sr concentration as well as with an increase in temperature. The multiple A-site ions in high-entropy rare-earth cobaltates result in an improved Seebeck coefficient ({\alpha}) compared to La$_{0.95}$Sr$_{0.05}$CoO$_3$, associated with a decrease in the Co-O-Co bond angle, which further enhances the power factor. The random distribution of cations at the rare-earth site results in a significant lowering of phonon thermal conductivity. As a result, a maximum figure of merit (zT) of 0.23 is obtained at 350K for (LaNdPrSmEu)$_{0.95}$Sr$_{0.05}$CoO$_3$, which is one of the highest values of zT reported at this temperature for oxide materials. This study shows promise to decouple thermoelectric parameters using the high-entropy concept in several materials.",2206.11106v1 2005-12-15,The WHO surveillance threshold and the emergence of drug-resistant HIV strains in Botswana,"Background: Approximately 40% of adults in Botswana are HIV-infected. The Botswana antiretroviral program began in 2002 and currently treats 34,000 patients with a goal of treating 85,000 patients (~30% of HIV-infected adults) by 2009. We predict the evolution of drug-resistant strains of HIV that may emerge as a consequence of this treatment program. We discuss the implications of our results for the World Health Organization's (WHO's) proposed surveillance system for detecting drug-resistant strains of HIV in Africa. Methods: We use a mathematical model of the emergence of drug resistance. We incorporate demographic and treatment data to make specific predictions as to when the WHO surveillance threshold is likely to be exceeded. Results: Our results show - even if rates of acquired resistance are high, but the drug-resistant strains that evolve are only half as transmissible as wild-type strains - that transmission of drug-resistant strains will remain low (< 5% by 2009) and are unlikely to exceed the WHO's surveillance threshold. However,our results show that transmission of drug-resistant strains in Botswana could increase to ~15% by 2009 if resistant strains are as transmissible as wild-type strains. Conclusion: The WHO's surveillance system is designed to detect transmitted resistance that exceeds a threshold level of 5%. Whether this system will detect drug-resistant strains in Botswana by 2009 will depend upon the transmissibility of the strains that emerge. Our results imply that it could be many years before the WHO detects transmitted resistance in other sub-Saharan African countries with less ambitious treatment programs than Botswana.",0512032v1 2020-04-10,Strain-engineering the Schottky barrier and electrical transport on MoS2,"Strain provides an effective means to tune the electrical properties while retaining the native chemical composition of the material. Unlike three-dimensional solids, two-dimensional materials withstand higher levels of elastic strain making it easier to tune various electrical properties to suit the technology needs. In this work we explore the effect of uniaxial tensile-strain on the electrical transport properties of bi- and few-layered MoS2, a promising 2D semiconductor. Raman shifts corresponding to the in-plane vibrational modes show a redshift with strain indicating a softening of the in-plane phonon modes. Photo luminescence measurements reveal a redshift in the direct and the indirect emission peaks signalling a reduction in the material bandgap. Transport measurements show a substantial enhancement in the electrical conductivity with a high piezoresistive gauge factor of ~ 321 superior to that for Silicon for our bi-layered device. The simulations conducted over the experimental findings reveal a substantial reduction of the Schottky barrier height at the electrical contacts in addition to the resistance of MoS2. Our studies reveal that strain is an important and versatile ingredient to tune the electrical properties of 2D materials and also can be used to engineer high-efficiency electrical contacts for future device engineering.",2004.05061v1 2011-08-25,"Synthesis, Crystal Growth and Epitaxial Layer Deposition of FeSe0.88 Superconductor and Other Poison Materials by Use of High Gas Pressure Trap System","The FeSe samples in the form of polycrystals, single crystals and thin films have been prepared and characterized. The synthesized material has been hot isostatically pressed under pressure of 0.45 GPa of 5N purity argon with the use of the high gas pressure trap system (HGPTS). Thin films have been fabricated by the mixed procedures with the use of DC sputtering from various types of targets and processed employing the HGPTS. The used HGPTS assures a full separation of the active volume for synthesis or crystal growth of material and the inert gas medium. The obtained FeSe0.88 samples have Tc between 8 and 12 K. The samples have been characterized by SEM, EDX, XRD, magnetic susceptibility and resistivity measurements.",1108.5069v1 2021-07-19,Making high-quality quantum microwave devices with van der Waals superconductors,"Ultra low-loss microwave materials are crucial for enhancing quantum coherence and scalability of superconducting qubits. Van der Waals (vdW) heterostructure is an attractive platform for quantum devices due to the single-crystal structure of the constituent two-dimensional (2D) layered materials and the lack of dangling bonds at their atomically sharp interfaces. However, new fabrication and characterization techniques are required to determine whether these structures can achieve low loss in the microwave regime. Here we report the fabrication of superconducting microwave resonators using NbSe$_2$ that achieve a quality factor $Q > 10^5$. This value sets an upper bound that corresponds to a resistance of $\leq 192 \mu\Omega$ when considering the additional loss introduced by integrating NbSe$_2$ into a standard transmon circuit. This work demonstrates the compatibility of 2D layered materials with high-quality microwave quantum devices.",2107.09147v3 2021-10-21,Phonon anharmonicity: a pertinent review of recent progress and perspective,"Anharmonic lattice vibrations govern the thermal dynamics in materials and present how the atoms interact and how they conduct heat. An indepth understanding of the microscopic mechanism of phonon anharmonicity in condensed systems is critical for developing better functional and energy materials. In recent years, a variety of novel behaviors in condense matters are driven by phonon anharmonic effects in some way or another, such as soft mode phase transition, negative thermal expansion, multiferroicity, ultralow thermal conductivity or high thermal resistance, and high-temperature superconductivity, etc. All these properties have endowed anharmonicity with many promising applications and provided remarkable opportunities for developing anharmonicity engineering, regulating heat transport towards excellent performance in materials. In this work, we review the recent development of the study on phonon anharmonic effect and summarize its origination, influence and mechanism, research methods, and applications. Besides, the remaining challenges, future trends, and prospects of phonon anharmonicity are also put forward.",2110.11094v1 2023-01-16,Nonlinear transport in a photo-induced superconductor,"Optically driven quantum materials exhibit a variety of non-equilibrium functional phenomena [1-11], which are potentially associated with unique transport properties. However, these transient electrical responses have remained largely unexplored, primarily because of the challenges associated with integrating quantum materials into ultrafast electrical devices. Here, thin films of K3C60 grown by Molecular Beam Epitaxy were connected by coplanar terahertz waveguides to a series of photo-conductive switches. This geometry enabled ultrafast transport measurements at high current densities, providing new information on the photo-induced phase created in the high temperature metal by mid-infrared excitation [12-16]. Nonlinearities in the current-voltage charactersitics of the transient state validate the assignment of transient superconductivity, and point to an inhomogeneous phase in which superconducting regions of the sample are connected by resistive weak links [17-23]. This work opens up the possibility of systematic transport measurements in driven quantum materials, both to probe their properties and to integrate them into ultrafast optoelectronic platforms.",2301.06425v1 2015-09-03,On the Concept of Cryptographic Quantum Hashing,"In the paper we define a notion of quantum resistant ($(\epsilon,\delta)$-resistant) hash function which combine together a notion of pre-image (one-way) resistance ($\epsilon$-resistance) property we define in the paper and the notion of collision resistance ($\delta$-resistance) properties. We show that in the quantum setting a one-way resistance property and collision resistance property are correlated: the ""more"" a quantum function is one-way resistant the ""less"" it collision resistant and vice versa. We present an explicit quantum hash function which is ""balanced"" one-way resistant and collision resistant and demonstrate how to build a large family quantum hash functions. Balanced quantum hash functions need a high degree of entanglement between the qubits. We use a ""phase constructions"" technique to express quantum hashing constructions, which is good to map hash states to coherent states in a superposition of time-bin modes. The later is ready to be implemented with current optical technology.",1509.01268v2 2019-12-11,Observation of excess resistance anomaly at resistive transitions in Ag/Au nanostructures,"The resistive transition in nanocomposite films of silver (Ag) nanoclusters of ~ 1 nm diameter embedded in gold (Au) matrix exhibits an anomalous resistance peak at the onset of the transition, even for transition temperatures as high as 260 K. The maximum value of the resistance ranges between ~ 30% - 300% above that of the normal state depending on devices as well as lead configuration within a single device. The excess resistance regime was observed in about 10% of the devices, and extends from ~ 10 - 100 K. Application of magnetic field of 9 T was found to partially suppress the excess resistance. From the critical current behavior, as well as negative differential resistance in the current-voltage characteristics, we discuss the possibility of interacting phase slip centers and alternate physical scenarios that may cause the excess resistance in our system.",1912.05428v1 2020-08-13,Properties of materials considered for improvised masks,"During a pandemic in which aerosol and droplet transmission is possible, the demand for masks that meet medical or workplace standards can prevent most individuals or organizations from obtaining suitable protection. Cloth masks are widely believed to impede droplet and aerosol transmission but most are constructed from materials with unknown filtration efficiency, airflow resistance and water resistance. Further, there has been no clear guidance on the most important performance metrics for the materials used by the general public (as opposed to high-risk healthcare settings). Here we provide data on a range of common fabrics that might be used to construct masks. None of the materials were suitable for masks meeting the N95 NIOSH standard, but many could provide useful filtration (>90%) of 3 micron particles (a plausible challenge size for human generated aerosols), with low pressure drop. These were: nonwoven sterile wraps, dried baby wipes and some double-knit cotton materials. Decontamination of N95 masks using isopropyl alcohol produces the expected increase in particle penetration, but for 3 micron particles, filtration efficiency is still well above 95%. Tightly woven thin fabrics, despite having the visual appearance of a good particle barrier, had remarkably low filtration efficiency and high pressure drop. These differences in filtration performance can be partly explained by the material structure; the better structures expose individual fibers to the flow while the poor materials may have small fundamental fibers but these are in tightly bundled yarns. The fit and use of the whole mask are critical factors not addressed in this work. Despite the complexity of the design of a very good mask, it is clear that for the larger aerosol particles, any mask will provide substantial protection to the wearer and those around them.",2008.06001v1 2022-06-01,A Pseudo-Two-Dimensional (P2D) Model for FeS2 Conversion Cathode Batteries,"Conversion cathode materials are gaining interest for secondary batteries due to their high theoretical energy and power density. However, practical application as a secondary battery material is currently limited by practical issues such as poor cyclability. To better understand these materials, we have developed a pseudo-two-dimensional model for conversion cathodes. We apply this model to FeS2 - a material that undergoes intercalation followed by conversion during discharge. The model is derived from the half-cell Doyle-Fuller-Newman model with additional loss terms added to reflect the converted shell resistance as the reaction progresses. We also account for polydisperse active material particles by incorporating a variable active surface area and effective particle radius. Using the model, we show that the leading loss mechanisms for FeS2 are associated with solid-state diffusion and electrical transport limitations through the converted shell material. The polydisperse simulations are also compared to a monodisperse system, and we show that polydispersity has very little effect on the intercalation behavior yet leads to capacity loss during the conversion reaction. We provide the code as an open-source Python Battery Mathematical Modelling (PyBaMM) model that can be used to identify performance limitations for other conversion cathode materials.",2206.00647v2 2024-03-12,Physics-Transfer Learning for Material Strength Screening,"The strength of materials, like many problems in the natural sciences, spans multiple length and time scales, and the solution has to balance accuracy and performance. Peierls stress is one of the central concepts in crystal plasticity that measures the strength through the resistance of a dislocation to plastic flow. The determination of Peierls stress involves a multiscale nature depending on both elastic lattice responses and the energy landscape of crystal slips. Material screening by strength via the Peierls stress from first-principles calculations is computationally intractable for the nonlocal characteristics of dislocations, and not included in the state-of-the-art computational material databases. In this work, we propose a physics-transfer framework to learn the physics of crystal plasticity from empirical atomistic simulations and then predict the Peierls stress from chemically accurate density functional theory-based calculations of material parameters. Notably, the strengths of single-crystalline metals can be predicted from a few single-point calculations for the deformed lattice and on the {\gamma} surface, allowing efficient, high-throughput screening for material discovery. Uncertainty quantification is carried out to assess the accuracy of models and sources of errors, showing reduced physical and system uncertainties in the predictions by elevating the fidelity of training models. This physics-transfer framework can be generalized to other problems facing the accuracy-performance dilemma, by harnessing the hierarchy of physics in the multiscale models of materials science.",2403.07526v1 2016-06-25,Observation of Optical and Electrical In-plane Anisotropy in High-mobility Few-layer ZrTe5,"Transition metal pentatelluride ZrTe5 is a versatile material in condensed-matter physics and has been intensively studied since the 1980s. The most fascinating feature of ZrTe5 is that it is a 3D Dirac semimetal which has linear energy dispersion in all three dimensions in momentum space. Structure-wise, ZrTe5 is a layered material held together by weak interlayer van der Waals force. The combination of its unique band structure and 2D atomic structure provides a fertile ground for more potential exotic physical phenomena in ZrTe5 related to 3D Dirac semimentals. However the physical properties of its few-layer form have yet to be thoroughly explored. Here we report strong optical and electrical in-plane anisotropy of mechanically exfoliated few-layer ZrTe5. Raman spectroscopy shows significant intensity change with sample orientations, and the behavior of angle-resolved phonon modes at the gamma point is explained by theoretical calculation. DC conductance measurement indicates a 50% of difference along different in-plane directions. The diminishing of resistivity anomaly in few-layer samples indicates the evolution of band structure with reduced thickness. Low-temperature Hall experiment sheds lights on more intrinsic anisotropic electrical transport, with hole mobility of 3,000 and 1,500 cm2/Vs along a-axis and c-axis respectively. Pronounced quantum oscillations in magneto-resistance are observed at low temperatures with highest electron mobility up to 44,000 cm2/Vs.",1606.07960v2 2018-09-25,Intrinsic Insulating Ground State in Transition Metal Dichalcogenide TiSe2,"The transition metal dichalcogenide TiSe$_2$ has received significant research attention over the past four decades. Different studies have presented ways to suppress the 200~K charge density wave transition, vary low temperature resistivity by several orders of magnitude, and stabilize magnetism or superconductivity. Here we give the results of a new synthesis technique whereby samples were grown in a high pressure environment with up to 180~bar of argon gas. Above 100~K, properties are nearly unchanged from previous reports, but a hysteretic resistance region that begins around 80~K, accompanied by insulating low temperature behavior, is distinct from anything previously observed. An accompanying decrease in carrier concentration is seen in Hall effect measurements, and photoemission data show a removal of an electron pocket from the Fermi surface in an insulating sample. We conclude that high inert gas pressure synthesis accesses an underlying nonmetallic ground state in a material long speculated to be an excitonic insulator.",1809.09467v2 2018-08-24,Data-driven Exploration of New Pressure-induced Superconductivity in PbBi$_2$Te$_4$ with Two Transition Temperatures,"Candidates compounds for new thermoelectric and superconducting materials, which have narrow band gap and flat bands near band edges, were exhaustively searched by the high-throughput first-principles calculation from an inorganic materials database named AtomWork. We focused on PbBi$_2$Te$_4$ which has the similar electronic band structure and the same crystal structure with those of a pressure-induced superconductor SnBi2Se4 explored by the same data-driven approach. The PbBi$_2$Te$_4$ was successfully synthesized as single crystals using a melt and slow cooling method. The core level X-ray photoelectron spectroscopy analysis revealed Pb2+, Bi3+ and Te2- valence states in PbBi$_2$Te$_4$. The thermoelectric properties of the PbBi$_2$Te$_4$ sample were measured at ambient pressure and the electrical resistivity was also evaluated under high pressure using a diamond anvil cell with boron-doped diamond electrodes. The resistivity decreased with increase of the pressure, and two pressure-induced superconducting transitions were discovered at 3.4 K under 13.3 GPa and at 8.4 K under 21.7 GPa. The data-driven approach shows promising power to accelerate the discovery of new thermoelectric and superconducting materials.",1808.07973v1 2021-03-17,Multi-level resistance switching and random telegraph noise analysis of nitride based memristors,"Resistance switching devices are of special importance because of their application in resistive memories (RRAM) which are promising candidates for replacing current nonvolatile memories and realize storage class memories. These devices exhibit usually memristive properties with many discrete resistance levels and implement artificial synapses. The last years, researchers have demonstrated memristive chips as accelerators in computing, following new in-memory and neuromorphic computational approaches. Many different metal oxides have been used as resistance switching materials in MIM or MIS structures. Understanding of the mechanism and the dynamics of resistance switching is very critical for the modeling and use of memristors in different applications. Here, we demonstrate the bipolar resistance switching of silicon nitride thin films using heavily doped Si and Cu as bottom and top-electrodes, respectively. Analysis of the current-voltage characteristics reveal that under space-charge limited conditions and appropriate current compliance setting, multi-level resistance operation can be achieved. Furthermore, a flexible tuning protocol for multi-level resistance switching was developed applying appropriate SET/RESET pulse sequences. Retention and random telegraph noise measurements performed at different resistance levels. The present results reveal the attractive properties of the examined devices.",2103.09931v1 2021-10-28,Spread and erase -- How electron hydrodynamics can eliminate the Landauer-Sharvin resistance,"It has long been realized that even a perfectly clean electronic system harbors a Landauer-Sharvin resistance, inversely proportional to the number of its conduction channels. This resistance is usually associated with voltage drops on the system's contacts to an external circuit. Recent theories have shown that hydrodynamic effects can reduce this resistance, raising the question of the lower bound of resistance of hydrodynamic electrons. Here we show that by a proper choice of device geometry, it is possible to spread the Landauer-Sharvin resistance throughout the bulk of the system, allowing its complete elimination by electron hydrodynamics. We trace the effect to the dynamics of electrons flowing in channels that terminate within the sample. For ballistic systems this termination leads to back-reflection of the electrons and creates resistance. Hydrodynamically, the scattering of these electrons off other electrons allows them to transfer to transmitted channels and avoid the resistance. Counter-intuitively, we find that in contrast to the ohmic regime, for hydrodynamic electrons the resistance of a device with a given width can decrease with its length, suggesting that a long enough device may have an arbitrarily small total resistance.",2110.15369v2 2005-08-04,Subharmonic gap structures and Josephson effect in MgB2/Nb micro-constrictions,"Superconducting micro-constrictions between Nb tips and high quality MgB$_{2}$ pellets have been realized by means of a point-contact inset, driven by a micrometric screw. Measurements of the current-voltage characteristics and of the dynamical conductance versus bias have been performed in the temperature range between 4.2 K and 500 K. Above the Nb critical temperature T$_{C}^{Nb}$, the conductance of the MgB$_2$/normal-metal constrictions behaves as predicted by the BTK model for low resistance contacts while high resistance junctions show quasiparticle tunneling characteristics. Consistently, from the whole set of data we infer the value $\Delta_{\pi} = 2.5 \pm 0.2$ meV for the three-dimensional gap of MgB$_2$. Below T$_{C}^{Nb}$, low resistance contacts show Josephson current and subharmonic gap structures (SGS), due to multiple Andreev reflections. Simultaneous observations of both features, unambiguously indicate coupling of the 3D band of MgB$_2$ with the Nb superconducting order parameter. We found that the temperature dependence of the Josephson critical current follows the classical Ambegaokar-Baratoff behavior with a value $I_CR_N=(2.1 \pm 0.1)$ meV at low temperatures.",0508137v2 2007-02-02,Dependence of electronic structure of SrRuO3 and the degree of correlation on cation off-stoichiometry,"We have grown and studied high quality SrRuO3 films grown by MBE as well as PLD. By changing the oxygen activity during deposition we were able to make SrRuO3 samples that were stoichiometric (low oxygen activity) or with ruthenium vacancies (high oxygen activity). Samples with strontium vacancies were found impossible to produce since the ruthenium would precipitate out as RuO2. The volume of the unit cell of SrRuO3 becomes larger as more ruthenium vacancies are introduced. The residual resistivity ratio (RRR) and room temperature resistivity were found to systematically depend on the volume of the unit cell and therefore on the amount of ruthenium vacancies. The RRR varied from ~30 for stoichiometric samples to less than two for samples that were very ruthenium poor. The room temperature resistivity varied from 190 microOhm cm for stoichoimetric samples to over 300 microOhm cm for very ruthenium poor samples. UPS spectra show a shift of weight from the coherent peak to the incoherent peak around the Fermi level when samples have more ruthenium vacancies. Core level XPS spectra of the ruthenium 3d lines show a strong screened part in the case of stoichiometric samples. This screened part disappears when ruthenium vacancies are introduced. Both the UPS and the XPS results are consistent with the view that correlation increases as the amount of ruthenium vacancies increase.",0702050v1 2007-11-17,Development of New Hole-Type Avalanche Detectors and the First Results of their Applications,"We have developed a new detector of photons and charged particles- a hole-type structure with electrodes made of a double layered resistive material: a thin low resistive layer coated with a layer having a much higher resistivity. One of the unique features of this detector is its capability to operate at high gas gains (up to 10E4) in air or in gas mixtures with air. They can also operate in a cascaded mode or be combined with other detectors, for example with GEM. This opens new avenues in their applications. Several prototypes of these devices based on new detectors and oriented on practical applications were developed and successfully tested: a detector of soft X-rays and alpha particles, a flame sensor, a detector of dangerous gases. All of these detectors could operate stably even in humid air and/or in dusty conditions. The main advantages of these detectors are their simplicity, low cost and high sensitivity. For example, due to the avalanche multiplication, the detectors of flames and dangerous gases have a sensitivity of 10-100 times higher than commercial devices. We therefore believe that new detectors will have a great future.",0711.2747v1 2010-10-29,Analytical method for parameterizing the random profile components of nanosurfaces imaged by atomic force microscopy,"The functional properties of many technological surfaces in biotechnology, electronics, and mechanical engineering depend to a large degree on the individual features of their nanoscale surface texture, which in turn are a function of the surface manufacturing process. Among these features, the surface irregularities and self-similarity structures at different spatial scales, especially in the range of 1 to 100 nm, are of high importance because they greatly affect the surface interaction forces acting at a nanoscale distance. An analytical method for parameterizing the surface irregularities and their correlations in nanosurfaces imaged by atomic force microscopy (AFM) is proposed. In this method, flicker noise spectroscopy - a statistical physics approach - is used to develop six nanometrological parameters characterizing the high-frequency contributions of jump- and spike-like irregularities into the surface texture. These contributions reflect the stochastic processes of anomalous diffusion and inertial effects, respectively, in the process of surface manufacturing. The AFM images of the texture of corrosion-resistant magnetite coatings formed on low-carbon steel in hot nitrate solutions with coating growth promoters at different temperatures are analyzed. It is shown that the parameters characterizing surface spikiness are able to quantify the effect of process temperature on the corrosion resistance of the coatings. It is suggested that these parameters can be used for predicting and characterizing the corrosion-resistant properties of magnetite coatings.",1010.6232v1 2013-04-04,Non-contact method for measurement of the microwave conductivity of graphene,"We report a non-contact method for conductivity and sheet resistance measurements of graphene samples using a high Q microwave dielectric resonator perturbation technique, with the aim of fast and accurate measurement of microwave conductivity and sheet resistance of monolayer and few layers graphene samples. The dynamic range of the microwave conductivity measurements makes this technique sensitive to a wide variety of imperfections and impurities and can provide a rapid non-contacting characterisation method. Typically the graphene samples are supported on a low-loss dielectric substrate, such as quartz, sapphire or SiC. This substrate is suspended in the near-field region of a small high Q sapphire puck microwave resonator. The presence of the graphene perturbs both centre frequency and Q value of the microwave resonator. The measured data may be interpreted in terms of the real and imaginary components of the permittivity, and by calculation, the conductivity and sheet resistance of the graphene. The method has great sensitivity and dynamic range. Results are reported for graphene samples grown by three different methods: reduced graphene oxide (GO), chemical vapour deposition (CVD) and graphene grown epitaxially on SiC. The latter method produces much higher conductivity values than the others.",1304.1304v1 2016-02-03,"Robust tunability of magnetorestance in Half-Heusler RPtBi (R = Gd, Dy, Tm, and Lu) compounds","We present the magnetic field dependencies of transport properties for $R$PtBi ($R$ = Gd, Dy, Tm, and Lu) half-Heusler compounds. Temperature and field dependent resistivity measurements of high quality $R$PtBi single crystals reveal an unusually large, non-saturating magnetoresistance (MR) up to 300 K under a moderate magnetic field of $H$ = 140 kOe. At 300 K, the large MR effect decreases as the rare-earth is traversed from Gd to Lu and the magnetic field dependence of MR shows a deviation from the conventional $H^{2}$ behavior. The Hall coefficient ($R_{H}$) for $R$ = Gd indicates a sign change around 120 K, whereas $R_{H}$ curves for $R$ = Dy, Tm, and Lu remain positive for all measured temperatures. At 300 K, the Hall resistivity reveals a deviation from the linear field dependence for all compounds. Thermoelectric power measurements on this family show strong temperature and magnetic field dependencies which are consistent with resistivity measurements. A highly enhanced thermoelectric power under applied magnetic field is observed as high as $\sim$100 $\mu$V/K at 140 kOe. Analysis of the transport data in this series reveals that the rare-earth-based Half-Husler compounds provide opportunities to tune MR effect through lanthanide contraction and to elucidate the mechanism of non-trivial MR.",1602.01194v1 2018-06-07,A Timing RPC with low resistive ceramic electrodes,"For precise start time determination a Beam Fragmentation T$_0$ Counter (BFTC) is under development for the Time-of-Flight Wall of the Compressed Baryonic Matter Spectrometer (CBM) at the Facility for Antiproton and Ion Research (FAIR) at Darmstadt/Germany. This detector will be located around the beam pipe, covering the front area of the Projectile Spectator Detector. The fluxes at this region are expected to exceed 10$^5$cm$^{-2}$s$^{-1}$. Resistive plate chambers (RPC) with ceramic composite electrodes could be use because of their high rate capabilities and radiation hardness of material. Efficiency $\ge$ 97\%, time resolution $\le$ 90 ps and rate capability $\ge$ 10$^5$cm$^{-2}$s$^{-1}$ were confirmed during many tests with high beam fluxes of relativistic electrons. We confirm the stability of these characteristics with low resistive Si$_3$N$_4$/SiC floating electrodes for a prototype of eight small RPCs, where each of them contains six gas gaps. The active RPC size amounts 20$\times$20 mm$^2$ produced on basis of Al$_3$O$_2$ and Si$_3$N$_4$/SiC ceramics. Recent test results obtained with relativistic electrons at the linear accelerator ELBE of the Helmholtz-Zentrum Dresden-Rossendorf with new PADI-10 Front-end electronic will be presented.",1806.02629v2 2019-05-07,Single-parameter scaling in the magnetoresistance of optimally doped La$_{2-x}$Sr$_{x}$CuO$_4$,"We show that the recent magnetoresistance data on thin-film La$_{2-x}$Sr$_{x}$CuO$_4$ (LSCO) in strong magnetic fields ($B$) obeys a single-parameter scaling of the form MR$(B,T)=f(\mu_H(T)B)$, where $\mu_H^{-1}(T)\sim T^{\alpha}$ ($1\le\alpha\le2$), from $T=180$K until $T\sim20$K, at which point the single-parameter scaling breaks down. The functional form of the MR is distinct from the simple quadratic-to-linear quadrature combination of temperature and magnetic field found in the optimally doped iron superconductor BaFe${}_2$(As${}_{1-x}$P${}_x$)${}_2$. Further, low-temperature departure of the MR in LSCO from its high-temperature scaling law leads us to conclude that the MR curve collapse is not the result of quantum critical scaling. We examine the classical effective medium theory (EMT) previously used to obtain the quadrature resistivity dependence on field and temperature for metals with a $T$-linear zero-field resistivity. It appears that this scaling form results only for a binary, random distribution of metallic components. More generally, we find a low-temperature, high-field region where the resistivity is simultaneously $T$ and $B$ linear when multiple metallic components are present. Our findings indicate that if mesoscopic disorder is relevant to the magnetoresistance in strange metal materials, the binary-distribution model which seems to be relevant to the iron pnictides is distinct from the more broad-continuous distributions relevant to the cuprates. Using the latter, we examine the applicability of classical effective medium theory to the MR in LSCO and compare calculated MR curves with the experimental data.",1905.02737v1 2021-01-18,Intrinsic hysteresis in the presumed superconducting transition of hydrides under high pressure,"Superconducting transitions in the absence of magnetic field should be non-hysteretic. Here we address the fact that the drops in electrical resistance that have been interpreted as evidence of superconductivity in several hydrides under high pressure (so-called ""superhydrides"") show hysteresis. We argue that the experimental evidence shows that the observed hysteresis cannot be attributed to experimental artifacts but is intrinsic to the samples. Assuming that the drops in resistance signal a thermodynamic phase transition, we argue that the presence of intrinsic thermal hysteresis indicates that these are first order transitions, whereas for standard superconductors the transition in the absence of applied magnetic field is always second order. We conclude that this is another feature that qualitatively distinguishes superhydrides from standard superconductors, in addition to the ones that have been pointed out earlier [1,2], $assuming$ these materials are superconductors. Alternatively and more likely, whether or not the drops in resistance signal a thermodynamic phase transition, our analysis indicates that superhydrides are not superconductors.",2101.07208v4 2021-03-27,Tesla's fluidic diode and the electronic-hydraulic analogy,"Reasoning by analogy is powerful in physics for students and researchers alike, a case in point being electronics and hydraulics as analogous studies of electric currents and fluid flows. Around 100 years ago, Nikola Tesla proposed a flow control device intended to operate similarly to an electronic diode, allowing fluid to pass easily in one direction but providing high resistance in reverse. Here we use experimental tests of Tesla's diode to illustrate principles of the electronic-hydraulic analogy. We design and construct a differential pressure chamber (akin to a battery) that is used to measure flow rate (current) and thus resistance of a given pipe or channel (circuit element). Our results prove the validity of Tesla's device, whose anisotropic resistance derives from its asymmetric internal geometry interacting with high-inertia flows, as quantified by the Reynolds number (here, Re ~ 1e3). Through the design and testing of new fluidic diodes, we explore the limitations of the analogy and the challenges of shape optimization in fluid mechanics. We also provide materials that may be incorporated into lesson plans for fluid dynamics courses, laboratory modules and further research projects.",2103.14813v1 2021-08-19,Measurement of the Low-temperature Loss Tangent of High-resistivity Silicon with a High Q-factor Superconducting Resonator,"In this letter, we present the direct loss tangent measurement of a high-resistivity intrinsic (100) silicon wafer in the temperature range from ~ 70 mK to 1 K, approaching the quantum regime. The measurement was performed using a technique that takes advantage of a high quality factor superconducting niobium resonator and allows to directly measure the loss tangent of insulating materials with high level of accuracy and precision. We report silicon loss tangent values at the lowest temperature and for electric field amplitudes comparable to those found in planar transmon devices one order of magnitude larger than what was previously estimated. In addition, we discover a non-monotonic trend of the loss tangent as a function of temperature that we describe by means of a phenomenological model based on variable range hopping conduction between localized states around the Fermi energy. We also observe that the dissipation increases as a function of the electric field and that this behavior can be qualitatively described by the variable range hopping conduction mechanism as well. This study lays the foundations for a novel approach to investigate the loss mechanisms and accurately estimate the loss tangent in insulating materials in the quantum regime, leading to a better understanding of coherence in quantum devices.",2108.08894v5 2007-06-01,High-Tc superconductivity originated from strong spin-charge correlation: indication from linear temperature dependence of resistivity,"Both the highest- and the linear temperature dependence of the resistivity in wide temperature range appear at the optimally doped regions of Cu-based superconductors1,2,3,4,5, and the highest- of Fe-based superconductors6,7 are also associated with the linear temperature dependence of the resistivity in normal states near superconducting states. This means that the high temperature superconductivity and the linear temperature dependence of the resistivity should be dominated by the same mechanism. This letter on theoretic calculation clearly shows that strong spin-charge correlation dominated resistivity behaves the linear temperature dependence, thus high-temperature superconductivity should be induced by strong spin-charge correlation.",0706.0059v2 2023-08-30,Investigation of W-SiC compositionally graded films as a divertor material,"W-SiC composite material is a promising plasma-facing material candidate alternative to pure W due to the low neutron activation, low impurity radiation, and low tritium diffusivity of SiC while leveraging the high erosion resistance of the W armor. Additionally, W and SiC have high thermomechanical compatibility given their similar thermal expansion rates. The present study addresses the synthesis and performance of compositionally graded W-SiC films fabricated by pulsed-DC magnetron sputtering. Compositional gradients were characterized using transmission electron microscopy (TEM) and energy-dispersive X-ray spectroscopy (EDS), and crystallographic information was obtained using electron diffraction and X-ray diffraction (XRD). Samples were exposed to L-mode deuterium plasma discharges in the DIII-D tokamak using the Divertor Material Evaluation System (DiMES). Post-mortem characterizations were performed using scanning electron microscopy (SEM) and XRD. Electron diffraction and XRD showed that the compositionally graded W-SiC films were composed of polycrystalline W and amorphous SiC with amorphous W+SiC interlayers. No macroscopic delamination or microstructural changes were observed under mild exposure conditions. This study serves as a preliminary examination of W-SiC compositionally graded composites as a potential candidate divertor material in future tokamak devices.",2308.16358v2 1999-09-28,"Magnetotransport properties of (Ga,Mn)As investigated at low temperature and high magnetic field","Magnetotransport properties of ferromagnetic semiconductor (Ga,Mn)As have been investigated. Measurements at low temperature (50 mK) and high magnetic field (<= 27 T) have been employed in order to determine the hole concentration p = 3.5x10^20 cm ^-3 of a metallic (Ga0.947Mn0.053)As layer. The analysis of the temperature and magnetic field dependencies of the resistivity in the paramagnetic region was performed with the use of the above value of p, which gave the magnitude of p-d exchange energy |N0beta | ~ 1.5 eV.",9909393v1 2003-09-28,Electron-Phonon Scattering in Metallic Single-Walled Carbon Nanotubes,"Electron scattering rates in metallic single-walled carbon nanotubes are studied using an atomic force microscope as an electrical probe. From the scaling of the resistance of the same nanotube with length in the low and high bias regimes, the mean free paths for both regimes are inferred. The observed scattering rates are consistent with calculations for acoustic phonon scattering at low biases and zone boundary/optical phonon scattering at high biases.",0309641v1 1998-10-26,High frequency magneto-impedance of double perovskite $La_{1.2}Sr_{1.8}Mn_{2}O_{7}$: secondary transitions at high temperatures,"Radio frequency magneto-impedance measurements clearly reveal a pronounced anomaly at 260K besides the main MI transition at 125K in the double perovskite material $La_{1.2}Sr_{1.8}Mn_{2}O_{7}$. This feature is not seen clearly in static resistivity and magnetization measurements. We suggest that this anomaly represents short range magnetic correlations enhanced at radio frequencies, with the easy axis along the c-axis .",9810351v2 1999-04-29,Consilience of High-Tc Theories,"Improvements both in the quality and in the variety of experiments on high-temperature superconductors have yielded new insights into the microscopic origins of pairing. A number of competing theories have already been ruled out. Some of the more promising descriptions -- gauge theories, coupled-chains, nesting instabilities, nodal liquids, and stripes -- share features in common. A unified picture of the cuprates is beginning to emerge.",9904437v1 1999-09-03,A thermostable trilayer resist for niobium lift-off,"We have developped a novel lift-off process for fabrication of high quality superconducting submicron niobium structures. The process makes use of a thermostable polymer with a high transition temperature T_{g}= 235 C and an excellent chemical stability. The superconducting critical temperature of 100 nm wide niobium lines is above 7 K. An example of shadow evaporation of a Nb-Cu submicron hybrid structure is given. A potential application of this process is the fabrication of very small single electron devices using refratory metals.",9909053v1 2003-10-29,Ultrasonic Defect Modification in Irradiated Silicon,"It is shown for the first time, that room temperature Ultrasonic Defect Manipulation (UDM) can significantly reduce the concentration of radiation defects in high resistivity silicon. Secondary Ion Mass Spectroscopy revealed that oxygen- and hydrogen- related chemical reactions in silicon are likely to occur under UDM at room temperature. Ultrasonically stimulated chemical reactions in solids can be an important source of energy, which is required for UDM.",0310675v1 2004-08-24,Barrier layer formation and PTCR effect in (1-x) Pb(Fe1/2Nb1/2)O3]-xPbTiO3 (x = 0.13) ceramics,"(1-x)Pb(Fe1/2Nb1/2)O3-PbTiO3(PFN-xPT)Ceramics with x = 0.13 sintered at 1473K show diffuse phase transition and very high dielectric constant at lower frequencies.The high value of dielectric constant at lower frequencies is shown to be due to the barrier layer formation.The resistivity of the PFN-xPT ceramics, obtained by complex impedance analysis, initially decreases with temperature and then shows an upward trend beyond the ferroelectric Curie point reminiscent of BaTiO3 based thermistors with PTCR effect.",0408509v1 2005-02-06,Model for a Macroscopically Disordered Conductor with an Exactly Linear High-Field Magnetoresistance,"We calculate the effective resistivity of a macroscopically disordered two dimensional conductor consisting of two components in a perpendicular magnetic field. When two components have equal area fractions, we use a duality theorem to show that the magnetoresistance is non-saturating and at high fields varies exactly linearly with magnetic field. At other compositions, an effective medium calculation leads to a saturating magnetoresistance. We briefly discuss possible connections between these results and magnetoresistance measurements on heavily disordered chalconide semiconductors.",0502162v2 2007-07-28,Performances of a Newly High Sensitive Trilayer F/Cu/F GMI Sensor,"We have selected stress-annealed nanocrystalline Fe-based ribbons for ferromagnetic/copper/ferromagnetic sensors exhibiting high magneto-impedance ratio. Longitudinal magneto-impedance reaches 400% at 60 kHz and longitudinal magneto-resistance increases up to 1300% around 200 kHz.",0707.4232v2 2009-09-25,Spin Injection Enhancement Through Schottky Barrier Superlattice Design,"We predict it is possible to achieve high-efficiency room-temperature spin injection from a mag- netic metal into InAs-based semiconductors using an engineered Schottky barrier based on an InAs/AlSb superlattice. The Schottky barrier with most metals is negative for InAs and positive for AlSb. For such metals there exist InAs/AlSb superlattices with a conduction band edge perfectly aligned with the metal's Fermi energy. The initial AlSb layer can be grown to the thickness required to produce a desired interface resistance. We show that the conductivity and spin lifetimes of such superlattices are sufficiently high to permit efficient spin injection from ferromagnetic metals.",0909.4594v1 2009-11-29,Current driven discontinuous insulator-metal transition and colossal low-field magnetoresistance in Sm0.6Sr0.4MnO3,"It is shown that with increasing magnitude of current (I), resistivity of Sm0.6Sr0.4MnO3 transforms from a smooth to a discontinuous insulator-metal transition which is also accompanied by an abrupt decrease in temperature of the sample. We report colossal low-field magnetoresistance under a high current bias (-99% at H = 0.5 T and 70 K) and electroresistance (-8000 % at H = 0 T and 60 K) for I = 11 mA. We interpret our observations in terms of current induced supercooling of the high temperature paramagnetic phase and enlargement of volume fraction of the ferromagnetic phase under a magnetic field.",0911.5491v1 2010-03-26,Superconductor terahertz metamaterial,"We characterize the behaviour of split ring resonators made up of high-transition temperature YBCO superconductor using terahertz time domain spectroscopy. The superconductor metamaterial shows sharp change in the transmission spectrum at the fundamental inductive-capacitive resonance and the dipole resonance as the temperature dips below the transition temperature. Our results reveal that the high performance of such a metamaterial is limited by material imperfections and defects such as cracks, voids and secondary phases which play dominant role in partially impeding the flow of current causing dissipation of energy and electrical resistance to appear in the superconductor film.",1003.5169v1 2013-08-15,Low Temperature Nanoscale Electronic Transport on the MoS_2 surface,"Two-probe electronic transport measurements on a Molybdenum Disulphide (MoS_2) surface were performed at low temperature (30K) under ultra-high vacuum conditions. Two scanning tunneling microscope tips were precisely positioned in tunneling contact to measure the surface current-voltage characteristics. The separation between the tips is controllably varied and measured using a high resolution scanning electron microscope. The MoS_2 surface shows a surface electronic gap (E_S) of 1.4eV measured at a probe separation of 50nm. Furthermore, the two- probe resistance measured outside the electronic gap shows 2D-like behavior with the two-probe separation.",1308.3299v1 2014-02-27,Nonlinear conductivity in CaRuO3 thin films measured by short current pulses,"Metals near quantum critical points have been predicted to display universal out-of equilibrium behavior in the steady current-carrying state. We have studied the non-linear conductivity of high-quality CaRuO$_3$ thin films with residual resistivity ratio up to 57 using micro-second short, high-field current pulses at low temperatures. Even for the shortest pulses of $5\mu$s, Joule heating persists, making it impossible to observe a possible universal non-linearity. Much shorter pulses are needed for the investigation of universal non-linear conductivity.",1402.6845v1 2015-02-02,Electrical and magnetic properties of La$_{0.5}$Rh$_4$Sb$_{12}$ filled skutterudite synthesized at high pressure,"A filled skutterudite, La$_{0.5}$Rh$_4$Sb$_{12}$, with a lattice constant of 9.284(2) {\AA} was synthesized using a high-pressure technique. The electrical resistivity showed semiconducting behavior and the energy gap was estimated to be more than 0.08 eV. Magnetic susceptibility measurements indicated temperature-independent diamagnetism, which originates from Larmor diamagnetism. The electrical properties of this compound are more similar to those of the La$_{0.5}$Rh$_4$As$_{12}$ semiconductor with an energy gap of 0.03 eV than to those of the La$_{0.6}$Rh$_4$P$_{12}$ superconductor.",1502.00337v2 2016-01-12,Melting of B12P2 boron subphosphide under pressure,"Melting of boron subphosphide (B12P2) to 26 GPa has been studied by in situ synchrotron X-ray powder diffraction in a laser-heated diamond anvil cell, and by quenching and electrical resistance measurements in a toroid-type high-pressure apparatus. B12P2 melts congruently, and the melting curve has a positive slope of 23(6) K/GPa. No solid-state phase transition was observed up to the melting in the whole pressure range under study.",1601.02930v1 2016-02-23,Preparation of Silver and Silver-backing self-supported thin targets by high vacuum evaporation,"We have produced in the Nuclear Physics Center in Lisbon thin film self-supported targets of Ag, LiF/Ag and CaF$_2$/Ag by a high vacuum resistance evaporation method. The production setup, materials, methods, characterization and results are described.",1602.07172v2 2016-05-09,Highly Non-linear and Reliable Amorphous Silicon Based Back-to-Back Schottky Diode as Selector Device for Large Scale RRAM Arrays,"In this work we present silicon process compatible, stable and reliable ($>10^{8}$cycles), high non-linearity ratio at half-read voltage ($>5\times 10^{5}$), high speed ($<60ns$) low operating voltage ($<2V$) back-to-back Schottky diodes. Materials choice of electrode, thickness of semiconductor layer and doping level are investigated by numerical simulation, experiments and current-voltage equations to give a general design consideration when back-to-back Schottky diodes are used as selector device for Resistive Random Access Memory(RRAM) arrays.",1605.02757v1 2016-07-19,Performance Enhancement of Black Phosphorus Field-Effect Transistors by Chemical Doping,"In this letter, a new approach to chemically dope black phosphorus (BP) is presented, which significantly enhances the device performance of BP field-effect transistors for an initial period of 18 h, before degrading to previously reported levels. By applying 2,3,5,6-tetrafluoro-7,7,8,8-tetracyanoquinodimethane (F4-TCNQ), low ON-state resistance of 3.2 ohm.mm and high field-effect mobility of 229 cm2/Vs are achieved with a record high drain current of 532 mA/mm at a moderate channel length of 1.5 {\mu}m.",1607.05760v1 2018-04-04,Ultra-high Vacuum Deposition of Higher Manganese Silicide Mn4Si7 Thin Films,"We have successfully grown one of the higher manganese silicides, Mn4Si7 thin films on silicon (100) substrates using an ultra-high vacuum deposition with a base pressure of 1x10-9 torr. The thickness of the film was varied from 65-100 nm. These films exhibit a tetragonal crystal structure and display paramagnetic behavior as predicted for the stoichiometric Mn4Si7 system. They have a resistivity of 3.321 x 10-5 ohm-m at room temperature and show a semi-metallic nature.",1804.01604v1 2018-04-09,Superconductivity in REO0.5F0.5BiS2 with high-entropy-alloy-type blocking layers,"We synthesized new REO0.5F0.5BiS2 (RE: rare earth) superconductors with the high-entropy-alloy-type (HEA-type) REO blocking layers. According to the RE concentration and the RE ionic radius, the lattice constant of a systematically changed in the HEA-type samples. A sharp superconducting transition was observed in the resistivity measurements for all the HEA-type samples, and the transition temperature of the HEA-type samples was higher than that of typical REO0.5F0.5BiS2. The sharp superconducting transition and the enhanced superconducting properties of the HEA-type samples may indicate the effectiveness of the HEA states of the REO blocking layers in the REO0.5F0.5BiS2 system.",1804.02880v2 2020-09-01,Solute softening and vacancy generation by diffusion-less climb in magnesium alloys,"Active room temperature diffusion-less climb of the edge dislocations in model Mg-Al alloys was observed using molecular dynamics simulations. Dislocations on prismatic and pyramidal I planes climb through the basal plane to overcome solute obstacles. This out-of-plane dislocation motion softens the high resistance pyramidal I glide and significantly reduces the anisotropy of dislocation mobility, and could help improve the ductility of Mg. The flow stress scales linearly with solute concentration, cAl. Dislocations climb predominantly in the negative direction, with climb angle on the order of 0.01cAl, producing very high vacancy concentration on the order of 10-4.",2009.00656v1 2020-06-20,Can an amorphous crystallize into a high entropy alloy?,"On the premise that amorphous-HEA composites could demonstrate high toughness and resistance to embrittlement akin to the phase separating glassy-solid solution composites, we develop a thermodynamics based approach to identify chemical compositions capable of undergoing the amorphous to HEA transformation. We introduce two new parameters called phase selection value (PSV) and molar volume dispersity parameter. Using this thermodynamic approach seven multi-component compositions were proposed and the general guidelines for identifying such compositions was established. The approach also reveals that BMGs may not be as such amenable to undergo an amorphous to HEA transformation.",2006.11579v1 2015-03-20,Bottom-up assembly of metallic germanium,"Extending chip performance beyond current limits of miniaturisation requires new materials and functionalities that integrate well with the silicon platform. Germanium fits these requirements and has been proposed as a high-mobility channel material,[1] a light emitting medium in silicon-integrated lasers,[2,3] and a plasmonic conductor for bio-sensing.[4,5] Common to these diverse applications is the need for homogeneous, high electron densities in three-dimensions (3D). Here we use a bottom-up approach to demonstrate the 3D assembly of atomically sharp doping profiles in germanium by a repeated stacking of two-dimensional (2D) high-density phosphorus layers. This produces high-density (10^19 to 10^20 cm-3) low-resistivity (10^-4 Ohmcm) metallic germanium of precisely defined thickness, beyond the capabilities of diffusion-based doping technologies.[6] We demonstrate that free electrons from distinct 2D dopant layers coalesce into a homogeneous 3D conductor using anisotropic quantum interference measurements, atom probe tomography, and density functional theory.",1503.05994v1 2014-08-06,Permanent magnet with MgB2 bulk superconductor,"Superconductors with persistent zero-resistance currents serve as permanent magnets for high-field applications requiring a strong and stable magnetic field, such as magnetic resonance imaging (MRI). The recent global helium shortage has quickened research into high-temperature superconductors (HTSs) materials that can be used without conventional liquid-helium cooling to 4.2 K. Herein, we demonstrate that 40-K-class metallic HTS magnesium diboride (MgB2) makes an excellent permanent bulk magnet, maintaining 3 T at 20 K for 1 week with an extremely high stability (<0.1 ppm/h). The magnetic field trapped in this magnet is uniformly distributed, as for single-crystalline neodymium-iron-boron. Magnetic hysteresis loop of the MgB2 permanent bulk magnet was detrmined. Because MgB2 is a simple-binary-line compound that does not contain rare-earth metals, polycrystalline bulk material can be industrially fabricated at low cost and with high yield to serve as strong magnets that are compatible with conventional compact cryocoolers, making MgB2 bulks promising for the next generation of Tesla-class permanent-magnet applications.",1408.1277v1 2014-08-20,In-situ hydrogen charging of zirconium powder to study isothermal percipitation of hydrides and determination of Zr-hydride crystal structure,"Zirconium alloys are widely used in the nuclear industry because of their high strength, good corrosion resistance and low neutron absorption cross-section. However, zirconium has strong affinity for hydrogen which leads to hydrogen concentration build-up over time. It is well known that the formation of hydrides will degrade the material and leads to, for example, delayed hydride cracking during high burn up. Even though zirconium hydrides have been studied for several decades, there still remain some controversies regarding the formation mechanisms, exact crystal structure, and stability of various hydride phases. This study uses high resolution synchrotron radiation as a probing tool to observe the precipitation and dissolution of hydrides in highly pure zirconium powder during in-situ hydrogen charging. The experiment enabled the direct observation of the hydride formation and phase transformations. It, also, provided high quality data for crystal structure determination.",1408.4665v1 2022-12-02,Ablation threshold and temperature dependent thermal conductivity of high entropy carbide thin films,"High entropy carbides (HECs) are a promising new class of ultra-high temperature ceramics that could provide novel material solutions for leading edges of hypersonic vehicles, which can reach temperatures above 3500C and experience extreme thermal gradients. Although the mechanical and thermal properties of HECs have been studied extensively at room temperature, few works have examined HEC properties at high temperatures or considered these materials' responses to thermal shock. In this work, we measure the thermal conductivity of a five-cation HEC up to 1200C. We find that thermal conductivity increases with temperature, consistent with trends demonstrated in single-metal carbides. We also measure thermal conductivity of an HEC deposited with varying CH4 flow rate, and find that although thermal conductivity is reduced when carbon content surpasses stoichiometric concentrations, the films all exhibited the same temperature dependent trends regardless of carbon content. To compare the thermal shock resistance of HECs with a refractory carbide, we conduct pulsed laser ablation measurements to determine the fluence threshold the HECs can withstand before damaging. We find that this metric for the average bond strength trends with the theoretical hardness of the HECs as expected.",2212.01238v1 2023-10-18,A New Class of Materials Based on Nanoporous High Entropy Alloys with Outstanding Properties,"Nanoporous metals with a random, bicontinuous structure of both pores and ligaments exhibit many unique mechanical properties, but their technical applications are often limited by their intrinsic brittleness under tensile strain triggered by fracture of the weakest ligaments. Here, we use molecular dynamics simulations to study the mechanical behavior and thermal stability of two different bicontinuous nanoporous high entropy alloys, Al0.1CoCrFeNi and NbMoTaW. To isolate the properties related to the nanoporous nature of our samples, we also studied the corresponding bulk and nanocrystalline systems. The results demonstrate that the specific modulus of nanoporous HEAs are 2 to 3 times greater than that of single element nanoporous materials with specific strength reaching values 5 to 10 times higher, comparable to bulk metals with the highest specific strength. Bicontinuous HEAs also displayed excellent resistance to thermal degradation as evidenced by the absence of coarsening ligaments up to temperatures of 1273 K which ensures the durability and reliability in high-temperature applications. The findings uncover unprecedented mechanical and thermal properties of bicontinuous nanoporous high entropy alloys, paving the way for their promising utilization in advanced engineering and structural applications.",2310.11937v1 1996-09-20,High Temperature Thermopower in La_{2/3}Ca_{1/3}MnO_3 Films: Evidence for Polaronic Transport,"Thermoelectric power, electrical resistivity and magnetization experiments, performed in the paramagnetic phase of La_{2/3}Ca_{1/3}MnO_3, provide evidence for polaron-dominated conduction in CMR materials. At high temperatures, a large, nearly field-independent difference between the activation energies for resistivity (rho) and thermopower (S), a characteristic of Holstein Polarons, is observed, and ln(rho) ceases to scale with the magnetization. On approaching T_c, both energies become field-dependent, indicating that the polarons are magnetically polarized. Below T_c, the thermopower follows a law S(H) prop. 1/rho (H) as in non saturated ferromagnetic metals.",9609212v1 2000-01-25,Influence of high-energy electron irradiation on the transport properties of La_{1-x}Ca_{x}MnO_{3} films (x \approx 1/3),"The effect of crystal lattice disorder on the conductivity and colossal magnetoresistance in La_{1-x}Ca_{x}MnO_{3} (x \approx 0.33) films has been examined. The lattice defects are introduced by irradiating the film with high-energy (\simeq 6 MeV) electrons with a maximal fluence of about 2\times 10^{17} cm^{-2}. This comparatively low dose of irradiation produces rather small radiation damage in the films. The number of displacements per atom (dpa) in the irradiated sample is about 10^{-5}. Nethertheless, this results in an appreciable increase in the film resistivity. The percentage of resistivity increase in the ferromagnetic metallic state (below the Curie tempetature T_{c}) was much greater than that observed in the insulating state (above T_{c}). At the same time irradiation has much less effect on T_{c} or on the magnitude of the colossal magnetoresistance. A possible explanation of such behavior is proposed.",0001372v1 2001-07-27,Lattice coupled first order magnetoresistance transition in an A-type antiferromagnet: Pr$_{0.46}$Sr$_{0.54}$MnO$_3$,"We investigated magnetic, magnetotransport and magnetostriction properties of the A-type antiferromagnet Pr$_{0.46}$Sr$_{0.54}$MnO$_3$ which undergoes a first order paramagnetic-antiferromagnetic transition below T$_N$ = 210 K while cooling and T$_N$ = 215 K while warming. The zero field ($\mu_0$H = 0 T) resistivity shows a sudden jump at T$_N$ and a small bump around T$_{max}$ = 220 K (\TEXTsymbol{>} T$_N$). T$_N$ shifts down and T$_{max}$ shifts up with increasing $\mu_0$H. Magnetoresistance as high as -45-57 % at 7 T is found in the temperature range 180 K-230 K. Isothermal measurements indicate that the field induced antiferromagnetic to ferromagnetic transition below T$_N$ is accompanied by a rapid decrease of the resistivity but increase of volume ($\Delta $V/V = +0.25 % at 180 K and 13.7 T). This lattice coupled magnetoresistance transition is suggested due to the field induced structural transition from the low volume orthorhombic to the high volume tetragonal structure.",0107560v1 2001-09-04,Magnetotransport in a bi-crystal film of La_0.7Sr_0.3MnO_3,"Transport properties of an epitaxial film of La_0.7Sr_0.3MnO_3 (LSMO), deposited epitaxially on a LaAlO_3 bi-crystal substrate having a misorientation angle of 9.2 deg., have been studied. The film was patterned into a meander containing 100 grain boundaries. The resistivity of the sample exhibits two components; one originating from the grain boundary regions, and one from the LSMO elements in the meander; the latter contribution is similar to the resistivity of a reference epitaxial LSMO film. The low (<0.5 T) and high (up to 6 T) field magnetoresistance was also studied. The meander show a large low field magnetoresistance, increasing with decreasing temperature, and a constant high field slope of the magnetoconductance, results that are well explained by a two-step spin polarized tunneling model.",0109052v1 2002-08-20,Fabrication and properties of gallium metallic photonic crystals,"Gallium metallic photonic crystals with 100% filling factor have been fabricated via infiltration of liquid gallium into opals of 300-nm silica spheres using a novel high pressure-high temperature technique. The electrical resistance of the Ga-opal crystals was measured at temperatures from 10 to 280 K. The data obtained show that Ga-opal crystals are metallic network with slightly smaller temperature coefficient of resistivity than that for bulk gallium. Optical reflectivity of bulk gallium, plain opal and several Ga-opal crystals were measured at photon energies from 0.3 to 6 eV. A pronounced photonic stop band in the visible spectral range was found in both the plain and Ga infiltrated opals. The reflectivity spectra also show increase in reflectivity below 0.6 eV; which we interpret as a significantly lower effective plasma frequency of the metallic mesh in the infiltrated opal compare to the plasma frequency in the pure metal.",0208392v1 2002-09-24,High Curie temperature GaMnAs obtained by resistance-monitored annealing,"We show that by annealing Ga1-xMnxAs thin films at temperatures significantly lower than in previous studies, and monitoring the resistivity during growth, an unprecedented high Curie temperature Tc and conductivity can be obtained. Tc is unambiguously determined to be 118 K for Mn concentration x=0.05, 140 K for x=0.06, and 120 K for x=0.08. We also identify a clear correlation between Tc and the room temperature conductivity. The results indicate that Curie temperatures significantly in excess of the current values are achievable with improvements in growth and post-growth annealing conditions.",0209554v1 2003-10-09,RF Surface Resistance of a HIPped MgB2 Sample at 21 GHz,"Magnesium diboride (MgB2) is attractive for RF cavity application for particle accelerators because it might not show an increase of RF surface losses at high magnetic surface fields, a phenomenon that has prevented high-Tc superconducting materials such as YBCO from being used for this application. We have measured the RF surface resistance (Rs) at 21 GHz of a MgB2 sample fabricated using Hot Isostatic Press (HIP) at 200 MPa and 1000 C. The results show that polishing with 0.1-micron diamond lapping film followed by a 1500-psi DI water rinse in a clean room reduced the Rs by a factor of 6.2 at 15 K and it is the lowest compared to other published data. The Rs data near the lowest temperature (~13 K) scatter between 0.6 and 1.3 mOhm. The penetration depth and energy gap were estimated to be 263 nm and 1.9-2.7, respectively, for the polished surface.",0310213v1 2004-08-31,"Normal state properties of high angle grain boundaries in (Y,Ca)Ba2Cu3O7-delta","By lithographically fabricating an optimised Wheatstone bridge geometry, we have been able to make accurate measurements of the resistance of grain boundaries in Y1-xCaxBa2Cu3O7-d between the superconducting transition temperature, Tc, and room temperature. Below Tc the normal state properties were assessed by applying sufficiently high currents. The behaviour of the grain boundary resistance versus temperature and of the conductance versus voltage are discussed in the framework charge transport through a tunnel barrier. The influence of misorientation angle, oxygen content, and calcium doping on the normal state properties is related to changes of the height and shape of the grain boundary potential barrier.",0409004v1 2005-07-06,"Oxidation Resistant Germanium Nanowires: Bulk Synthesis, Long Chain Alkanethiol Functionalization and Langmuir-Blodgett Assembly","A simple method is developed to synthesize gram quantities of uniform Ge nanowires (GeNWs) by chemical vapor deposition on preformed, monodispersed seed-particles loaded onto high surface area silica support. Various chemical functionalization schemes are investigated to passivate the GeNW surfaces using alkanethiols and alkyl Grignard reactions. The stability of functionalization against oxidation of germanium for various alkyl chain lengths is elucidated by X-ray photoelectron spectroscopy. Among all schemes tested, long chain alkanethiols (>=C12) are found to impart the most stable GeNW passivation against oxidation upon extended exposure to ambient air. Further, the chemically functionalized oxidation-resistant nanowires are soluble in organic solvents and can be readily assembled into close-packed Langmuir-Blodgett films potentially useful for future high performance electronic devices.",0507145v2 2006-03-08,Nanoscopic processes of Current Induced Switching in thin tunnel junctions,"In magnetic nanostructures one usually uses a magnetic field to commute between two resistance (R) states. A less common but technologically more interesting alternative to achieve R-switching is to use an electrical current, preferably of low intensity. Such Current Induced Switching (CIS) was recently observed in thin magnetic tunnel junctions, and attributed to electromigration of atoms into/out of the insulator. Here we study the Current Induced Switching, electrical resistance, and magnetoresistance of thin MnIr/CoFe/AlO$_x$/CoFe tunnel junctions. The CIS effect at room temperature amounts to 6.9% R-change between the high and low states and is attributed to nanostructural rearrangements of metallic ions in the electrode/barrier interfaces. After switching to the low R-state some electro-migrated ions return to their initial sites through two different energy channels. A low (high) energy barrier of $\sim$0.13 eV ($\sim$0.85 eV) was estimated. Ionic electromigration then occurs through two microscopic processes associated with different types of ions sites/defects. Measurements under an external magnetic field showed an additional intermediate R-state due to the simultaneous conjugation of the MR (magnetic) and CIS (structural) effects.",0603208v1 2007-04-13,Counting and manipulating single electrons using a carbon nanotube transistor,"We report on the electric measurements of an individual Au nanoparticle with an ultra-high contact resistance of about $10^{19} \Omega$. The high-impedance measurements have been carried out by counting the electrons that are transferred onto the particle. In order to do this, a carbon nanotube is used as the electrode for the supply of electrons but also as the detector of the charge transfer. Measurements using single-electron detection allow us to determine the separation between the electron states in the Au nanoparticle, which is about 4 meV, consistent with the charging energy of the particle. Single-electron detection with nanotubes offers great promise for the study of electron transfer in highly resistive molecular systems.",0704.1794v1 2007-07-17,Positive and negative pressure effects on the magnetic ordering and the Kondo effect in the compound Ce2RhSi3,"The competition between magnetic ordering and the Kondo effect in Ce2RhSi3, ordering antiferromagnetically at 7 K, is investigated by the measurements of magnetization, heat capacity and electrical resistivity on the solid solutions, Ce(2-x)La(x)RhSi3, Ce(2-y)Y(y)RhSi3, and Ce2RhSi(3-z)Ge(z), as well as by high pressure studies on this compound. The trends in the Kondo and Neel temperature variations among these alloys are compared to infer the roles of unit-cell volume and electronic structure changes. On the basis of the results, we infer that this compound lies at the peak of Doniach-magnetic-phase-diagram. The high pressure electrical resistivity data indicate that the quantum critical point for this compound is in the vicinity of 4 GPa.",0707.2518v1 2007-09-05,Thickness-dependence of the electronic properties in V2O3 thin films,"High quality vanadium sesquioxide V2O3 films (170-1100 {\AA}) were grown using the pulsed laser deposition technique on (0001)-oriented sapphire substrates, and the effects of film thickness on the lattice strain and electronic properties were examined. X-ray diffraction indicates that there is an in-plane compressive lattice parameter (a), close to -3.5% with respect to the substrate and an out-of-plane tensile lattice parameter (c) . The thin film samples display metallic character between 2-300 K, and no metal-to-insulator transition is observed. At low temperature, the V2O3 films behave as a strongly correlated metal, and the resistivity (\rho) follows the equation \rho =\rho_0 + A T^2, where A is the transport coefficient in a Fermi liquid. Typical values of A have been calculated to be 0.14 \mu\Omega cm K^{-2}, which is in agreement with the coefficient reported for V2O3 single crystals under high pressure. Moreover, a strong temperature-dependence of the Hall resistance confirms the electronic correlations of these V2O3 thin films samples.",0709.0692v1 2008-06-09,Superconductivity in single crystals of LaFePO,"Single crystals of the compound LaFePO were prepared using a flux growth technique at high temperatures. Electrical resistivity measurements reveal metallic behavior and a resistive transition to the superconducting state at a critical temperature T_c ~ 6.6 K. Magnetization measurements also show the onset of superconductivity near 6 K. In contrast, specific heat measurements manifest no discontinuity at T_c. These results lend support to the conclusion that the superconductivity is associated with oxygen vacancies that alter the carrier concentration in a small fraction of the sample, although superconductivity characterized by an unusually small gap value can not be ruled-out. Under applied magnetic fields, T_c is suppressed anisotropically for fields perpendicular and parallel to the ab-plane, suggesting that the crystalline anisotropy strongly influences the superconducting state. Preliminary high-pressure measurements show that T_c passes through a maximum of nearly 14 K at ~ 110 kbar, demonstrating that significantly higher T_c values may be achieved in the phosphorus-based oxypnictides.",0806.1265v2 2009-08-23,Superconductivity at high Tc in neodymium-doped 1111-SrFeAsF system,"Polycrystalline Sr1-xNdxFeAsF samples were prepared at various Nd-doping levels using both a stoichiometric mixture of the starting materials and in slight excess amounts of FeAs. Susceptibility and resistivity of the samples were studied down to 4 K revealing a probable coexistence of superconductivity and a magnetic ordering. Temperature dependence of resistivity for all the Nd-doped samples shows the presence of a transition below 15 K most likely originating from the magnetic ordering of Nd moments, while the spin-density-wave anomaly at 175 K survives up to 0.35 Nd-doping. Superconductivity only occurs above 0.40 Nd-doping with onset maximum Tc reaching as high as 52 K.",0908.3285v3 2011-06-29,Hysteretic magnetoresistance and thermal bistability in a magnetic two-dimensional hole system,"Colossal negative magnetoresistance and the associated field-induced insulator-to-metal transition, the most characteristic features of magnetic semiconductors, are observed in n-type rare earth oxides and chalcogenides, p-type manganites, n-type and p-type diluted magnetic semiconductors (DMS) as well as in quantum wells of n-type DMS. Here, we report on magnetostransport studies of Mn modulation-doped InAs quantum wells, which reveal a magnetic field driven and bias voltage dependent insulator-to-metal transition with abrupt and hysteretic changes of resistance over several orders of magnitude. These phenomena coexist with the quantised Hall effect in high magnetic fields. We show that the exchange coupling between a hole and the parent Mn acceptor produces a magnetic anisotropy barrier that shifts the spin relaxation time of the bound hole to a 100 s range in compressively strained quantum wells. This bistability of the individual Mn acceptors explains the hysteretic behaviour while opening prospects for information storing and processing. At high bias voltage another bistability, caused by the overheating of electrons10, gives rise to abrupt resistance jumps.",1106.5832v1 2011-09-06,Evolution of transport properties of BaFe2-xRuxAs2 in a wide range of isovalent Ru substitution,"The effects of isovalent Ru substitution at the Fe sites of BaFe2-xRuxAs2 are investigated by measuring resistivity and Hall coefficient on high-quality single crystals in a wide range of doping (0 < x < 1.4). Ru substitution weakens the antiferromagnetic (AFM) order, inducing superconductivity for relatively high doping level of 0.4 < x < 0.9. Near the AFM phase boundary, the transport properties show non-Fermi-liquid-like behaviors with a linear-temperature dependence of resistivity and a strong temperature dependence of Hall coefficient with a sign change. Upon higher doping, however, both of them recover conventional Fermi-liquid behaviors. Strong doping dependence of Hall coefficient together with a small magnetoresistance suggest that the anomalous transport properties can be explained in terms of anisotropic charge carrier scattering due to interband AFM fluctuations rather than a conventional multi-band scenario.",1109.1083v1 2012-09-06,High-temperature thermoelectric properties of the double-perovskite ruthenium oxide (Sr$_{1-x}$La$_x$)$_2$ErRuO$_6$,"We have prepared polycrystalline samples of (Sr$_{1-x}$La$_x$)$_2$ErRuO$_6$ and (Sr$_{1-x}$La$_x$)$_2$YRuO$_6$, and have measured the resistivity, Seebeck coefficient, thermal conductivity, susceptibility and x-ray absorption in order to evaluate the electronic states and thermoelectric properties of the doped double-perovskite ruthenates. We have observed a large Seebeck coefficient of -160 $\mu$V/K and a low thermal conductivity of 7 mW/cmK for $x$=0.1 at 800 K in air. These two values are suitable for efficient oxide thermoelectrics, although the resistivity is still as high as 1 $\Omega$cm. From the susceptibility and x-ray absorption measurements, we find that the doped electrons exist as Ru$^{4+}$ in the low spin state. On the basis of the measured results, the electronic states and the conduction mechanism are discussed.",1209.1250v1 2012-10-12,Simultaneous measurement of pressure evolution of crystal structure and superconductivity in FeSe0.92 using designer diamonds,"Simultaneous high pressure x-ray diffraction and electrical resistance measurements have been carried out on a PbO type {\alpha}-FeSe0.92 compound to a pressure of 44 GPa and temperatures down to 4 K using designer diamond anvils at synchrotron source. At ambient temperature, a structural phase transition from a tetragonal (P4/nmm) phase to an orthorhombic (Pbnm) phase is observed at 11 GPa and the Pbnm phase persists up to 74 GPa. The superconducting transition temperature (TC) increases rapidly with pressure reaching a maximum of ~28 K at ~ 6 GPa and decreases at higher pressures, disappearing completely at 14.6 GPa. Simultaneous pressure-dependent x-ray diffraction and resistance measurements at low temperatures show superconductivity only in a low pressure orthorhombic (Cmma) phase of the {\alpha}-FeSe0.92. Upon increasing pressure at 10 K near TC, crystalline phases change from a mixture of orthorhombic (Cmma) and hexagonal (P63/mmc) to a high pressure orthorhombic (Pbnm) phase near 6.4 GPa where TC is maximum.",1210.3645v1 2012-11-20,Optically excited multi-band conduction in LaAlO3/SrTiO3 heterostructures,"The low-temperature resistance of a conducting LaAlO3/SrTiO3 interface with a 10 nm thick LaAlO3 film decreases by more than 50% after illumination with light of energy higher than the SrTiO3 band-gap. We explain our observations by optical excitation of an additional high mobility electron channel, which is spatially separated from the photo-excited holes. After illumination, we measure a strongly non-linear Hall resistance which is governed by the concentration and mobility of the photo-excited carriers. This can be explained within a two-carrier model where illumination creates a high-mobility electron channel in addition to a low-mobility electron channel which exists before illumination.",1211.4778v1 2013-12-04,Physical characteristics and cation distribution of NiFe2O4 thin films with high resistivity prepared by reactive co-sputtering,"We fabricated NiFe2O thin films on MgAl2O4 (001) substrates by reactive dc magnetron co-sputtering in a pure oxygen atmosphere at different substrate temperatures. The film properties were investigated by various techniques with a focus on their structure, surface topography, magnetic characteristics, and transport properties. Structural analysis revealed a good crystallization with epitaxial growth and low roughness and a similar quality as in films grown by pulsed laser deposition. Electrical conductivity measurements showed high room temperature resistivity (12 Ohmm), but low activation energy, indicating an extrinsic transport mechanism. A band gap of about 1.55 eV was found by optical spectroscopy. Detailed x-ray spectroscopy studies confirmed the samples to be ferrimagnetic with fully compensated Fe moments. By comparison with multiplet calculations of the spectra we found that the cation valencies are to a large extent Ni2+ and Fe3+.",1312.1086v1 2013-12-13,Low-energy electronic properties of clean CaRuO$_3$: elusive Landau quasiparticles,"We have prepared high-quality epitaxial thin films of CaRuO$_3$ with residual resistivity ratios up to 55. Shubnikov-de Haas oscillations in the magnetoresistance and a $T^2$ temperature dependence in the electrical resistivity only below 1.5 K, whose coefficient is substantially suppressed in large magnetic fields, establish CaRuO$_3$ as a Fermi liquid (FL) with anomalously low coherence scale. Non-Fermi liquid (NFL) $T^{3/2}$ dependence is found between 2 and 25 K. The high sample quality allows access to the intrinsic electronic properties via THz spectroscopy. For frequencies below 0.6 THz, the conductivity is Drude-like and can be modeled by FL concepts, while for higher frequencies non-Drude behavior, inconsistent with FL predictions, is found. This establishes CaRuO$_3$ as a prime example of optical NFL behavior in the THz range.",1312.3809v1 2017-10-18,Near-thermal limit gating in heavily-doped III-V semiconductor nanowires using polymer electrolytes,"Doping is a common route to reducing nanowire transistor on-resistance but has limits. High doping level gives significant loss in gate performance and ultimately complete gate failure. We show that electrolyte gating remains effective even when the Be doping in our GaAs nanowires is so high that traditional metal-oxide gates fail. In this regime we obtain a combination of sub-threshold swing and contact resistance that surpasses the best existing p-type nanowire MOSFETs. Our sub-threshold swing of 75 mV/dec is within 25% of the room-temperature thermal limit and comparable with n-InP and n-GaAs nanowire MOSFETs. Our results open a new path to extending the performance and application of nanowire transistors, and motivate further work on improved solid electrolytes for nanoscale device applications.",1710.06950v2 2018-02-02,Magneto-transport properties of proposed triply degenerate topological semimetal Pd$_{3}$Bi$_{2}$S$_{2}$,"We report transport properties of single-crystalline Pd$_{3}$Bi$_{2}$S$_{2}$, which has been predicted to host an unconventional electronic phase of matter beyond three-dimensional Dirac and Weyl semimetals. Similar to several topological systems, the resistivity shows field induced metal-semiconductor-like crossover at low temperature. Large, anisotropic and non-saturating magnetoresistance (MR) has been observed in transverse experimental configuration. At 2 K and 9 T, the MR value reaches as high as $\sim$1.1$\times$10$^{3}$ \%. Hall resistivity reveals the presence of two types of charge carriers and has been analyzed using two-band model. In spite of the large density ($>$ 10$^{21}$ cm$^{-3}$), the mobility of charge carriers is found to be quite high ($\sim$ 0.75$\times$10$^{4}$ cm$^{2}$ V$^{-1}$ s$^{-1}$ for hole and $\sim$ 0.3$\times$10$^{4}$ cm$^{2}$ V$^{-1}$ s$^{-1}$ for electron). The observed magneto-electrical properties indicate that Pd$_{3}$Bi$_{2}$S$_{2}$ may be a new member of the topological semimetal family, which can have a significant impact in technological applications.",1802.00712v2 2019-09-17,Spin-Orbit-Torque Field-Effect Transistor (SOTFET): Proposal for a New Magnetoelectric Memory,"Spin-based memories are attractive for their non-volatility and high durability but provide modest resistance changes, whereas semiconductor logic transistors are capable of large resistance changes, but lack memory function with high durability. The recent availability of multiferroic materials provides an opportunity to directly couple the change in spin states of a magnetic memory to a charge change in a semiconductor transistor. In this work, we propose and analyze the spin-orbit torque field-effect transistor (SOTFET), a device with the potential to significantly boost the energy efficiency of spin-based memories, and to simultaneously offer a palette of new functionalities.",1909.08133v3 2017-03-09,Transport properties of iron at the Earth's core conditions: the effect of spin disorder,"The electronic and thermal transport properties of the Earth's core are crucial for many geophysical models such as the geodynamo model of the Earth's magnetic field and of its reversals. Here we show, by considering bcc-iron and iron-rich iron-silicon alloy as a representative of the Earth's core composition and applying the first-principles modeling that the spin disorder at the Earth's core conditions provides an essential contribution, of order 20~$\mu\Omega$\,cm, to the electrical resistivity. This value is comparable in magnitude with the electron-phonon and with the recently estimated electron-electron scattering contributions. The origin of the spin-disorder resistivity (SDR) consists in the existence of fluctuating local moments that are stabilized at high temperatures by the magnetic entropy even at pressures at which the ground state of iron is non-magnetic. We find that electron-phonon and SDR contributions are not additive at high temperatures. We thus observe a large violation of the Matthiessen rule, not common in conventional metallic alloys at ambient conditions.",1703.03205v3 2020-04-07,Large-scalable fabrication of improved Bi-Te-based flexible thermoelectric modules using a semiconductor manufacturing process,"Among the several flexible thermoelectric modules in existence, sintered Bi-Te-based modules represent a viable option because of their high output power density and flexibility, which enables the use of arbitrary heat sources. We have fabricated Bi-Te-based modules with a large-scalable fabrication process and improved their output performance. The reduction in the interconnection resistance, using thick electrodes of the flexible printed circuit, significantly improves the module's output power to 87 mW/cm$^{2}$ at $\Delta T$ = 70 K, which is 1.3-fold higher than a previous prototype module. Furthermore, the establishment of the fabrication for the top electrodes by using the surface mount technology makes it possible to realize a high-throughput manufacturing of the module. Our durability tests reveal that there is no significant change in the internal resistance of the module during 10000 cycles of mechanical bending test and 1000 cycles of thermal stress test.",2004.03068v1 2020-09-24,Pressure-Temperature Phase Diagram of $α$-Mn,"Electrical resistivity and ac-susceptibility measurements under high pressure were carried out in high-quality single crystals of $\alpha$-Mn. The pressure-temperature phase diagram consists of an antiferromagnetic ordered phase (0<$P$<1.4 GPa, $T$ 365 days. We have tested the chamber for its long term operation. The leakage current, bulk resistivity, efficiency, noise rate and time resolution of the chamber have been found to be quite stable during the testing peroid. It showed an efficiency $>$ 95$\%$ with an average time resolution of $\sim$0.83 ns at the point of measurement at 9000 V throughout the testing period. Details of the long term performance of the chamber have been discussed.",1604.03668v2 2016-07-25,Influencia del potencial de polarización en la deposición de películas delgadas de NiO,"Nickel oxide (NiO) is a binary compound with a lot of applications in the present technology. NiO thin films were deposited by reactive sputtering magnetron under several voltage biases applied in the glass substrates (0, 50, 100, 200, 300, 400 and 500 V). Films were characterized by profilometry, X-ray diffraction, elemental composition and electrical resistivity at room temperature and at low temperatures. The present work showed that despite the insulating behavior of substrate the residual stress was reduced at high biases and the (111) texture was promoted. Electrical resistivity was reduced at high bias and at low temperatures thermal activation of p-type conduction was detected.",1607.07391v1 2017-01-29,Built-in Homojunction Dominated Intrinsically Rectifying-Resistive Switching in NiO Nanodots for Selection Device-Free Memory Application,"The intrinsically rectifying-resistive switching (IR-RS) has been regarded as an effective way to address the crosstalk issue, due to the Schottky diodes formed at the metal/oxide interfaces in the ON states to suppress the sneak current at reverse biases. In this letter, we report for the first time another type of IR-RS that is related to the built-in homojunction. The IR-RS study was usually limited to macroscopic samples with micron-order pad-type electrodes, while this work is on NiO nanodots fabricated with ultrathin anodic-aluminum-oxide templates and acting as nanoscaled analogs of real devices. The NiO nanodots show high storage density and high uniformity, and the IR-RS behaviors are of good device performances in terms of retention, endurance, switching ratio and rectification ratio. The feasibility of the IR-RS for selection device-free memory application has been demonstrated, by calculating the maximum crossbar array size under the worst-case scenario to be 3 Mbit.",1702.05665v1 2018-02-20,Perturbation theories behind thermal mode spectroscopy for high-accuracy measurement of thermal diffusivity of solids,"Thermal mode spectroscopy (TMS) has been recently proposed for accurately measuring thermal diffusivity of solids from a temperature decay rate of a specific thermal mode selected by three- dimensional (anti)nodal information [Phys. Rev. Lett., 117, 195901 (2016)]. In this paper, we find out the following advantages of TMS by use of perturbation analyses. First, TMS is applicable to the measurement of high thermal diffusivity with a small size specimen. Second, it is less affected by thermally resistive films on a specimen in the sense that the resistance at the interface does not affect the first-order correction of thermal diffusivity. Third, it can perform doubly accurate measurement of the thermal diffusivity specified at a thermal equilibrium state even if the diffusivity depends on temperature in the sense that the measurement can be performed within tiny temperature difference from the given state and that the decay rate of the slowest decaying mode is not affected by the dependence.",1802.07378v2 2020-02-28,Hydrodynamic and ballistic transport over large length scales in GaAs/AlGaAs,"We study hydrodynamic and ballistic transport regimes through nonlocal resistance measurements and high-resolution kinetic simulations in a mesoscopic structure on a high-mobility two-dimensional electron system in a GaAs/AlGaAs heterostructure. We evince the existence of collective transport phenomena in both regimes and demonstrate that negative nonlocal resistances and current vortices are not exclusive to only the hydrodynamic regime. The combined experiments and simulations highlight the importance of device design, measurement schemes and one-to-one modeling of experimental devices to demarcate various transport regimes.",2002.12806v3 2019-03-07,Fe-Sn nanocrystalline films for flexible magnetic sensors with high thermal stability,"The interplay of magnetism and spin-orbit coupling on an Fe kagome lattice in Fe3Sn2 crystal produces a unique band structure leading to an order of magnitude larger anomalous Hall effect than in conventional ferromagnetic metals. In this work, we demonstrate that Fe-Sn nanocrystalline films also exhibit a large anomalous Hall effect, being applicable to magnetic sensors that satisfy both high sensitivity and thermal stability. In the films prepared by a co-sputtering technique at room temperature, the partial development of crystalline lattice order appears as nanocrystals of Fe-Sn kagome layer. The tangent Hall angle, the ratio of Hall resistivity to longitudinal resistivity, is largely enhanced in the optimal alloy composition of close to Fe3Sn2, exemplifying the kagome origin even though the films are composed of nanocrystal and amorphous-like domains. These ferromagnetic Fe-Sn films possess great advantages as a Hall sensor over semiconductors in thermal stability owing to the weak temperature dependence of the anomalous Hall responses. Moreover, the room-temperature fabrication enables us to develop a mechanically flexible Hall sensor on an organic substrate. These demonstrations manifest the potential of kagome metal as an untapped reservoir for designing new functional devices.",1903.02689v1 2021-01-25,Statics and Dynamics of Space-Charge-Layers in Polarized Inorganic Solid Electrolytes,"The quest for safe high-energy batteries with ""5V-class"" cathodes and lithium metal anodes drives research into solid electrolytes. However, reasons for the large charge transfer resistances -- the major bottleneck of all-solid-state batteries -- are still debated. In this article, we explore the processes in incompressible solid electrolytes between blocking electrodes by theory-based continuum modeling and numerical simulations. We investigate the experimentally observed wide space-charge-zones in solid electrolytes, which are a possible cause for the high interfacial resistances. On time scales relevant for battery applications, we reduce our model equations. Analytic and numeric calculations predict and study the actual structure of space-charge-layers in solid electrolytes. To illustrate these dynamics and validate our model, computational results are presented and compared with experimental observations. Analog to semiconductors, we determine the material dependent, asymmetric space-charge-layer width in the low temperature limit approximately. This allows us to make an explicit statement about the influence of defect concentrations and dielectric properties on the width of the space-charge-layers in homogeneous solid electrolytes.",2101.10294v1 2015-06-01,High-pressure study of the Weyl semimetal NbAs,"We performed a series of high-pressure synchrotron X-ray diffraction (XRD) and resistance measurements on the Weyl semimetal NbAs. The crystal structure remains stable up to 26 GPa according to the powder XRD data. The resistance of NbAs single crystal increases monotonically with pressure at low temperature. Up to 20 GPa, no superconducting transition is observed down to 0.3 K. These results show that the Weyl semimetal phase is robust in NbAs, and applying pressure is not a good way to get a topological superconductor from a Weyl semimetal.",1506.00374v2 2020-08-14,High-Mobility Carriers Induced by Chemical Doping in the Candidate Nodal-Line Semimetal CaAgP,"We report the electronic properties of single crystals of candidate nodal-line semimetal CaAgP. The transport properties of CaAgP are understood within the framework of a hole-doped nodal-line semimetal. In contrast, Pd-doped CaAgP shows a drastic increase of magnetoresistance at low magnetic fields and a strong decrease of electrical resistivity at low temperatures probably due to weak antilocalization. Hall conductivity data indicated that the Pd-doped CaAgP has not only hole carriers induced by the Pd doping, but also high-mobility electron carriers in proximity of the Dirac point. Electrical resistivity of Pd-doped CaAgP also showed a superconducting transition with onset temperature of 1.7-1.8 K.",2008.06188v1 2020-12-19,Anomalous behavior in high-pressure carbonaceous sulfur hydride,"A new experimental study by Snider et al. [Nature 586, 373-377 (2020)] reported behavior in a high-pressure carbon-sulfur-hydrogen system that has been interpreted by the authors as superconductivity at room temperature. The sudden drop of electrical resistance at a critical temperature and the change of the R vs. T behavior with an applied magnetic field point to superconductivity. This is a very exciting study in one of the most important areas of science, hence, it is crucial for the community to investigate these findings and hopefully reproduce these results. In this comment, we present calculations that expand upon the arguments put forth by Hirsch and Marsiglio [arXiv:2010.10307], and offer some speculations about physical mechanisms that might explain the observed data. In agreement with Hirsch and Marsiglio, we show that there are errors in the analysis presented in the experimental paper, and with the correct analysis, the reported R vs. T data significantly deviate from the expected behavior. In particular, the extremely sharp change in resistance at the superconducting transition is not consistent with a strongly type II superconductor.",2012.10771v3 2021-02-23,High magnetic field induced crossover from the Kondo to Fermi liquid behavior in 1$T$-VTe$_{2}$ single crystals,"The magnetic and magnetotransport properties of metallic 1$T$-VTe$_{2}$ single crystals were investigated at temperatures from 1.3 to 300 K and in magnetic fields up to 35 T. Upon applying a high magnetic field, it is found that the electrical resistivity displays a crossover from the logarithmic divergence of the single-impurity Kondo effect to the Fermi liquid behavior at low temperatures. The Brillouin scale of the negative magnetoresistivity above the Kondo temperature $T_{\rm{K}}$ = 12 K indicates that the Kondo features originate from intercalated V ions, with $S$ = 1/2. Both magnetic susceptibility and Hall effect show an anomaly around $T_{\rm{K}}$. By using the modified Hamann expression we successfully describe the temperature-dependent resistivity under various magnetic fields, which shows the characteristic peak below $T_{\rm{K}}$ due to the splitting of the Kondo resonance.",2102.11444v1 2021-02-26,Crossover from itinerant to localized states in the thermoelectric oxide [Ca$_2$CoO$_3$]$_{0.62}$[CoO$_2$],"The layered cobaltite [Ca$_2$CoO$_3$]$_{0.62}$[CoO$_2$], often expressed as the approximate formula Ca$_3$Co$_4$O$_9$, is a promising candidate for efficient oxide thermoelectrics but an origin of its unusual thermoelectric transport is still in debate. Here we investigate \textit{in-plane} anisotropy of the transport properties in a broad temperature range to examine the detailed conduction mechanism. The in-plane anisotropy between $a$ and $b$ axes is clearly observed both in the resistivity and the thermopower, which is qualitatively understood with a simple band structure of the triangular lattice of Co ions derived from the angle-resolved photoemission spectroscopy experiments. On the other hand, at high temperatures, the anisotropy becomes smaller and the resistivity shows a temperature-independent behavior, both of which indicate a hopping conduction of localized carriers. Thus the present observations reveal a crossover from low-temperature itinerant to high-temperature localized states, signifying both characters for the enhanced thermopower.",2102.13250v1 2021-11-03,Devices for Thermal Conductivity Measurements of Electroplated Bi for X-ray TES Absorbers,"Electroplated Bismuth (Bi) is commonly used in Transition-Edge Sensors (TESs) for X-rays because of its high stopping power and low heat capacity. Electroplated Bi is usually grown on top of another metal that acts as seed layer, typically gold (Au), making it challenging to extrapolate its thermoelectric properties. In this work, we present four-wire resistance measurement structures that allow us to measure resistance as a function of temperature of electroplated Bi independently of Au. The results show that the thermal conductivity of the Bi at 3 K is high enough to guarantee the correct thermalization of X-ray photons when used as an absorber for TESs.",2111.02503v1 2021-11-09,Absence of decoherence in the electron-wall system,"Decoherence is associated with a dissipative environment as described by the Caldeira-Leggett equation. Anglin and Zurek predicted that a resistive surface could act as such a dissipative environment for a free electron wave passing close to it. We scrutinize Zurek's and other promising decoherence theoretical models by observing electrons passing by an optically excited GaAs surface and through a gold channel. The high resistivity of the GaAs surface and close proximity to the gold surface leads to strong decoherence within these decoherence models. In contradistinction, the observed contrast is high in our electron diffraction patterns. This implies lower decoherence rates than suggested by these models, making electron-matter-wave-guides and other technologies, where quantum coherence of electrons close to materials is important, a possibility",2111.05246v1 2022-06-10,Fabrication of uniformly doped graphene quantum Hall arrays with multiple quantized resistance outputs,"In this work, limiting factors for developing metrologically useful arrays from epitaxial graphene on SiC are lifted with a combination of centimeter-scale, high-quality material growth and the implementation of superconducting contacts. Standard devices for metrology have been restricted to having a single quantized value output based on the $\nu$ = 2 Landau level. With the demonstrations herein of devices having multiple outputs of quantized values available simultaneously, these versatile devices can be used to disseminate the ohm globally. Such devices are designed to give access to quantized resistance values over the range of three orders of magnitude, starting as low as the standard value of approximately 12.9 k$\Omega$ and reaching as high as 1.29 M$\Omega$. Several experimental methods are used to assess the quality and versatility of the devices, including standard lock-in techniques and Raman spectroscopy.",2206.05098v1 2022-06-29,On the depletion behaviour of low-temperature covalently bonded silicon sensor diodes,"Low temperature covalent direct wafer-wafer bonding allows for the fusion of multiple semiconductor wafers without any additional material at the bonding interface. In the context of particle pixel detectors this might provide an alternative to bump-bonding for joining sensors to readout chips. Previous investigations have shown that the amorphous layer formed at the interface during bonding is detrimental to charge propagation. To investigate the influence of the bonding interface on signal collection we have fabricated custom test structures by bonding high-resistivity N to high-resistivity P-type silicon wafers thus forming P-N junctions. Scanning transmission electron microscopy shows indeed the formation of ca. 3nm wide amorphous layer at the interface. Using a scanning transient current technique (TCT) setup we were able to record generated signals. Illuminating our sample with light of different wavelengths and from different sides, indicates that the P side of the bonded structures can be fully depleted, but not the N side. This indicates a strongly asymmetric depletion behaviour which we attribute to the presence of the bonding interface.",2206.14717v2 2022-07-26,Engineering Surface Oxygen Vacancies in $\mathrm{SrTiO_3}$ to Form a High Mobility and Transparent Quasi Two dimensional Electron System,"Quasi-two-dimensional electron systems (q-2DES) are formed in various hetero-structures, including oxide interfaces. Oxygen vacancies (OVs) in oxides like $\mathrm{SrTiO_3}$ are known to produce electronic carriers. A novel way to produce $\mathrm{SrTiO_{3-\delta}}$ on the surface using a low-energy $\mathrm{H_2}$ plasma is shown here. It results in a q-2DES with mobility as high as $\mu \sim 20,000 \; cm^2V^{-1}s^{-1}$, displaying quantum oscillations in magneto-resistance. We can achieve a sharper or weaker confinement potential by adjusting the process pressure. The system with sharper confinement displays clearer quantum oscillations and Kondo-like temperature dependence of resistance. OVs close to the surface behaving like a correlated Anderson impurity is responsible for the Kondo behaviour. Quantum oscillations are less prominent in the weakly confined system. A cross-over from weak-localization to anti-localization with temperature is seen, but no Kondo behavior. The process also results in a transparent conductor amenable to lithographic patterning. This conductor's standard figure of merit is comparable to poly-crystalline ITO films in the visible regime and extends with similar performance into the $\lambda$ $\sim 1.5$ $\mu m$ telecommunication wavelength.",2207.12933v1 2022-09-05,Growth of rare-earth monopnictide DySb single crystal by novel Self-flux method,"This report presents a new synthesis protocol for the single crystal growth of rare earth monopnictide DySb by self-flux technique. A detailed structural, transport and magnetic characterization have been done using X-Ray diffraction (XRD), High resolution X-Ray diffraction (HRXRD), resistivity and magnetization measurements respectively. The Rietveld refinement of powder XRD pattern confirms that the grown crystal is in single phase and crystallizes in space group Fm3m(225) of rock-salt type crystal structure. HRXRD on cleaved crystal confirms the single crystalline nature while rocking curve analysis reveals the high quality of the grown crystal. Temperature dependent resistivity and magnetization measurements show a transition at 9.7K from paramagnetic (PM) to antiferromagnetic (AFM) state.",2209.01930v1 2022-10-27,Single photon detection performance of highly disordered NbTiN thin films,"We experimentally investigated the detection performance of highly disordered NbxTi1-xN based superconducting nanowire single photon detectors (SNSPDs). The dependence on the composition of the transition temperature Tc for NbxTi1-xN films show a dome-like behavior on the Nb content, with a maximal Tc at xNb~0.65 , and the Nb0.65Ti0.35N films also combine relatively large sheet resistance and intermediate residual resistivity ratio. Moreover, 60-nm-wide and 7-nm-thick Nb0.65Ti0.35N nanowires show a switching current as high as 14.5 uA, and saturated intrinsic detection efficiency with a plateau of more than 2 uA at 2.4 K. Finally, the corresponding SNSPDs on an alternative SiO2/Ta2O5 dielectric mirror showed a system detection efficiency of approximately 92% for 1550 nm photons, and the timing jitter is around 26 ps. Our results demonstrate that the highly disordered NbxTi1-xN films are promising for fabricating SNSPDs for near- and middle-infrared single photons with high detection efficiency and low timing jitter.",2210.15215v1 2022-11-24,Development of Hybrid Resistive Plate Chambers,"Resistive Plate Chambers (RPCs) are essential active media of large-scale experiments as part of the muon systems and (semi-)digital hadron calorimeters. Among the several outstanding issues associated with the RPCs, the loss of efficiency for the detection of particles when subjected to high particle fluxes, and the limitations associated with the common RPC gases can be listed. In order to address the latter issue, we developed novel RPC designs with special anode plates coated with high secondary electron emission yield materials such as Al$_2$O$_3$ and TiO$_2$. The proof of principle was obtained for various designs and is in progress for the rest. The idea was initiated following the achievements on the development of the novel 1-glass RPCs. Here we report on the construction of various different RPC designs, and their performance measurements in laboratory tests and with particle beams; and discuss the future test plans.",2211.13796v2 2023-09-11,Experimental realization of a high Curie temperature CoFeRuSn quaternary Heusler alloy for spintronic applications,"We synthesize CoFeRuSn equiatomic quaternary Heusler alloy using arc-melt technique and investigate its structural, magnetic and transport properties. The room temperature powder X-ray diffraction analysis reveals that CoFeRuSn crystallizes in cubic crystal structure with small amount of DO3 - disorder. The field dependence of magnetization shows non-zero but small hysteresis and saturation behavior up to room temperature, indicating soft ferromagnetic nature of CoFeRuSn. The magnetic moment estimated from the magnetization data is found to be 4.15 {\mu}B / f.u., which is slightly less than the expected Slater-Pauling rule. The deviation in the value of experimentally observed moment from the theoretical value might be due to small disorder in the crystal. The low temperature fit to electrical resistivity data show absence of quadratic temperature dependence of resistivity, suggesting half-metallic behavior of CoFeRuSn. The high Curie temperature and possible half-metallic behavior of CoFeRuSn make it a highly promising candidate for room temperature spintronic applications.",2309.05493v1 2018-04-11,Extremely large magnetoresistance in topologically trivial semimetal $α$-WP$_2$,"Extremely large magnetoresistance (XMR) was recently discovered in many non-magnetic materials, while its underlying mechanism remains poorly understood due to the complex electronic structure of these materials. Here, we report an investigation of the $\alpha$-phase WP$_2$, a topologically trivial semimetal with monoclinic crystal structure (C2/m), which contrasts to the recently discovered robust type-II Weyl semimetal phase in $\beta$-WP$_2$. We found that $\alpha$-WP$_2$ exhibits almost all the characteristics of XMR materials: the near-quadratic field dependence of MR, a field-induced up-turn in resistivity following by a plateau at low temperature, which can be understood by the compensation effect, and high mobility of carriers confirmed by our Hall effect measurements. It was also found that the normalized MRs under different magnetic fields has the same temperature dependence in $\alpha$-WP$_2$, the Kohler scaling law can describe the MR data in a wide temperature range, and there is no obvious change in the anisotropic parameter $\gamma$ value with temperature. The resistance polar diagram has a peanut shape when field is rotated in $\textit{ac}$ plane, which can be understood by the anisotropy of Fermi surface. These results indicate that both field-induced-gap and temperature-induced Lifshitz transition are not the origin of up-turn in resistivity in the $\alpha$-WP$_2$ semimetal. Our findings establish $\alpha$-WP$_2$ as a new reference material for exploring the XMR phenomena.",1804.03879v1 2019-05-02,Robust axion insulator and Chern insulator phases in a two-dimensional antiferromagnetic topological insulator,"The intricate interplay between nontrivial topology and magnetism in two-dimensional (2D) materials has led to the emergence of many novel phenomena and functionalities. An outstanding example is the quantum anomalous Hall (QAH) effect, which was realized in magnetically doped topological insulators (TIs) in the absence of magnetic field. Recently, the layered van der Waals compound MnBi2Te4 has been theoretically predicted and experimentally verified to be a TI with interlayer antiferromagnetic (AFM) order. It is a rare stoichiometric material with coexisting topology and magnetism, thus represents a perfect building block for complex topological-magnetic structures. Here we investigate the quantum transport behaviors of both bulk crystal and exfoliated MnBi2Te4 flakes in a field effect transistor geometry. In the 6 septuple layers (SLs) device tuned into the insulating regime, we observe a large longitudinal resistance and zero Hall plateau, which are characteristic of the axion insulator state. The robust axion insulator state occurs in zero magnetic field, over a wide magnetic field range, and at relatively high temperatures. Moreover, a moderate magnetic field drives a quantum phase transition from the axion insulator phase to a Chern insulator phase with zero longitudinal resistance and quantized Hall resistance h/e2 (h is the Plank constant and e is the elemental charge). These results pave the road for using even-number-SL MnBi2Te4 to realize the quantized topological magnetoelectric effect and axion electrodynamics in condensed matter systems.",1905.00715v2 2019-04-24,Antisymmetric magnetoresistance in van der Waals Fe3GeTe2/graphite/Fe3GeTe2 tri-layer heterostructures,"Van der Waals (vdW) ferromagnetic materials are rapidly establishing themselves as effective building blocks for next generation spintronic devices. When layered with non-magnetic vdW materials, such as graphene and/or topological insulators, vdW heterostructures can be assembled (with no requirement for lattice matching) to provide otherwise unattainable device structures and functionalities. We report a hitherto rarely seen antisymmetric magnetoresistance (MR) effect in van der Waals heterostructured Fe3GeTe2/graphite/Fe3GeTe2 devices. Unlike conventional giant magnetoresistance (GMR) which is characterized by two resistance states, the MR in these vdW heterostructures features distinct high, intermediate and low resistance states. This unique characteristic is suggestive of underlying physical mechanisms that differ from those observed before. After theoretical calculations, the three resistance behavior was attributed to a spin momentum locking induced spin polarized current at the graphite/FGT interface. Our work reveals that ferromagnetic heterostructures assembled from vdW materials can exhibit substantially different properties to those exhibited by similar heterostructures grown in vacuum. Hence, it highlights the potential for new physics and new spintronic applications to be discovered using vdW heterostructures.",1904.10588v2 2007-03-09,Nanometer-Scale Materials Contrast Imaging with a Near-Field Microwave Microscope,"We report topography-free materials contrast imaging on a nano-fabricated Boron-doped Silicon sample measured with a Near-field Scanning Microwave Microscope over a broad frequency range. The Boron doping was performed using the Focus Ion Beam technique on a Silicon wafer with nominal resistivity of 61 Ohm.cm. A topography-free doped region varies in sheet resistance from 1000Ohm/Square to about 400kOhm/Square within a lateral distance of 4 micrometer. The qualitative spatial-resolution in sheet resistance imaging contrast is no worse than 100 nm as estimated from the frequency shift signal.",0703241v1 2010-03-15,A Memadmittance Systems Model for Thin Film Memory Materials,"In 1971 the memristor was originally postulated as a new non-linear circuit element relating the time integrals of current and voltage. More recently researchers at HPLabs have linked the theoretical memristor concept to resistance switching behavior of TiO(2-x) thin films. However, a variety of other thin film materials exhibiting memory resistance effects have also been found to exhibit a memory capacitance effect. This paper proposes a memadmittance (memory admittance) systems model which attempts to consolidate the memory capacitance effects with the memristor model. The model produces equations relating the cross-sectional area of conductive bridges in resistive switching films to shifts in capacitance.",1003.2842v1 2018-09-06,Estimation of the electrical and thermal contact resistances and thermoemf of thermoelectric material-metal transient contact layer due to semiconductor surface rougness,"The impact of semiconductor surface roughness on the electrical and thermal contact resistances and thermoEMF of thermoelectric material (TEM)-metal transient contact layer is studied theoretically. The distribution of hollows and humps on the rough surface is simulated by the truncated Gaussian distribution. The impact of distribution parameters on the electrical contact resistance and thermoEMF of thermoelectric material-metal contact is studied.",1809.02504v1 2022-03-30,STeP-CiM: Strain-enabled Ternary Precision Computation-in-Memory based on Non-Volatile 2D Piezoelectric Transistors,"We propose 2D Piezoelectric FET (PeFET) based compute-enabled non-volatile memory for ternary deep neural networks (DNNs). PeFETs consist of a material with ferroelectric and piezoelectric properties coupled with Transition Metal Dichalcogenide channel. We utilize (a) ferroelectricity to store binary bits (0/1) in the form of polarization (-P/+P) and (b) polarization dependent piezoelectricity to read the stored state by means of strain-induced bandgap change in Transition Metal Dichalcogenide channel. The unique read mechanism of PeFETs enables us to expand the traditional association of +P (-P) with low (high) resistance states to their dual high (low) resistance depending on read voltage. Specifically, we demonstrate that +P (-P) stored in PeFETs can be dynamically configured in (a) a low (high) resistance state for positive read voltages and (b) their dual high (low) resistance states for negative read voltages, without afflicting a read disturb. Such a feature, which we name as Polarization Preserved Piezoelectric Effect Reversal with Dual Voltage Polarity (PiER), is unique to PeFETs and has not been shown in hitherto explored memories. We leverage PiER to propose a Strain-enabled Ternary Precision Computation-in-Memory (STeP-CiM) cell with capabilities of computing the scalar product of the stored weight and input, both of which are represented with signed ternary precision. Further, using multi word-line assertion of STeP-CiM cells, we achieve massively parallel computation of dot products of signed ternary inputs and weights. Our array level analysis shows 91% lower delay and improvements of 15% and 91% in energy for in-memory multiply-and-accumulate operations compared to near-memory design approaches based on SRAM and PeFET respectively. STeP-CiM exhibits upto 8.91x improvement in performance and 6.07x average improvement in energy over SRAM/PeFET based near-memory design.",2203.16416v1 2013-01-28,Can high risk fungicides be used in mixtures without selecting for fungicide resistance?,"Fungicide mixtures produced by the agrochemical industry often contain low-risk fungicides, to which fungal pathogens are fully sensitive, together with high-risk fungicides known to be prone to fungicide resistance. Can these mixtures provide adequate disease control while minimizing the risk for the development of resistance? We present a population dynamics model to address this question. We found that the fitness cost of resistance is a crucial parameter to determine the outcome of competition between the sensitive and resistant pathogen strains and to assess the usefulness of a mixture. If fitness costs are absent, then the use of the high-risk fungicide in a mixture selects for resistance and the fungicide eventually becomes nonfunctional. If there is a cost of resistance, then an optimal ratio of fungicides in the mixture can be found, at which selection for resistance is expected to vanish and the level of disease control can be optimized.",1301.6561v2 2005-12-15,Introduction to tensorial resistivity probability tomography,"The probability tomography approach developed for the scalar resistivity method is here extended to the 2D tensorial apparent resistivity acquisition mode. The rotational invariant derived from the trace of the apparent resistivity tensor is considered, since it gives on the datum plane anomalies confined above the buried objects. Firstly, a departure function is introduced as the difference between the tensorial invariant measured over the real structure and that computed for a reference uniform structure. Secondly, a resistivity anomaly occurrence probability (RAOP) function is defined as a normalised crosscorrelation involving the experimental departure function and a scanning function derived analytically using the Frechet derivative of the electric potential for the reference uniform structure. The RAOP function can be calculated in each cell of a 3D grid filling the investigated volume, and the resulting values can then be contoured in order to obtain the 3D tomographic image. Each non-vanishing value of the RAOP function is interpreted as the probability which a resistivity departure from the reference resistivity obtain in a cell as responsible of the observed tensorial apparent resistivity dataset on the datum plane. A synthetic case shows that the highest RAOP values correctly indicate the position of the buried objects and a very high spacial resolution can be obtained even for adjacent objects with opposite resistivity contrasts with respect to the resistivity of the hosting matrix. Finally, an experimental field case dedicated to an archaeological application of the resistivity tensor method is presented as a proof of the high resolution power of the probability tomography imaging, even when the data are collected in noisy open field conditions.",0512147v1 2014-07-24,Macro- and microscopic properties of strontium doped indium oxide,"Solid state synthesis and physical mechanisms of electrical conductivity variation in polycrystalline, strontium doped indium oxide In2O3:(SrO)x were investigated for materials with different doping levels at different temperatures (T=20-300 C) and ambient atmosphere content including humidity and low pressure. Gas sensing ability of these compounds as well as the sample resistance appeared to increase by 4 and 8 orders of the magnitude, respectively, with the doping level increase from zero up to x=10%. The conductance variation due to doping is explained by two mechanisms: acceptor-like electrical activity of Sr as a point defect and appearance of an additional phase of SrIn2O4. An unusual property of high level (x=10%) doped samples is a possibility of extraordinarily large and fast oxygen exchange with ambient atmosphere at not very high temperatures (100-200 C). This peculiarity is explained by friable structure of crystallite surface. Friable structure provides relatively fast transition of samples from high to low resistive state at the expense of high conductance of the near surface layer of the grains. Microscopic study of the electro-diffusion process at the surface of oxygen deficient samples allowed estimation of the diffusion coefficient of oxygen vacancies in the friable surface layer at room temperature as 3x10^(-13) cm^2/s, which is by one order of the magnitude smaller than that known for amorphous indium oxide films.",1407.6471v1 2015-03-29,Universal low-temperature Ohmic contacts for quantum transport in transition metal dichalcogenides,"Low carrier mobility and high electrical contact resistance are two major obstacles prohibiting explorations of quantum transport in TMDCs. Here, we demonstrate an effective method to establish low-temperature Ohmic contacts in boron nitride encapsulated TMDC devices based on selective etching and conventional electron-beam evaporation of metal electrodes. This method works for most extensively studied TMDCs in recent years, including MoS2, MoSe2, WSe2, WS2, and 2H-MoTe2. Low electrical contact resistance is achieved at 2 K. All of the few-layer TMDC devices studied show excellent performance with remarkably improved field-effect mobilities ranging from 2300 cm2/V s to 16000 cm2/V s, as verified by the high carrier mobilities extracted from Hall effect measurements. Moreover, both high-mobility n-type and p-type TMDC channels can be realized by simply using appropriate contact metals. Prominent Shubnikov-de Haas oscillations have been observed and investigated in these high-quality TMDC devices.",1503.08427v2 2017-04-13,"High-pressure phase diagram, structural transitions, and persistent non-metallicity of BaBiO$_3$: theory and experiment","BaBiO$_3$ is a mixed-valence perovskite which escapes the metallic state through a Bi valence (and Bi-O bond) disproportionation or CDW distortion, resulting in a semiconductor with a gap of 0.8 eV at zero pressure. The evolution of structural and electronic properties at high pressure is, however, largely unknown. Pressure, one might have hoped, could reduce the disproportionation, making the two Bi ions equivalent and bringing the system closer to metallicity or even to superconductivity, such as is attained at ambient pressure upon metal doping. We address the high-pressure phase diagram of pristine BaBiO$_3$ by ab initio DFT calculations based on GGA and hybrid functionals in combination with crystal structure prediction methods based on evolutionary algorithms, molecular dynamics and metadynamics. The calculated phase diagram from 0 to 50 GPa indicates that pristine BaBiO$_3$ resists metallization under pressure, undergoing instead at room temperature structural phase transitions from monoclinic \textit{I2/m} to nearly tetragonal \textit{P-1} at 7 GPa, possibly to monoclinic \textit{C2/m} at 27 GPa, and to triclinic \textit{P1} at 43 GPa. Remarkably, all these phases sustain and in fact increase the inequivalence of two Bi neighboring sites and of their Bi-O bonds and, in all cases except semimetallic \textit{C2/m}, the associated insulating character. We then present high-pressure resistivity data which generally corroborate these results, and show that the insulating character persists at least up to 80 GPa, suggesting that the \textit{C2/m} phase is probably an artifact of the small computational cell.",1704.04098v1 2019-11-18,Effect of particle contact on the electrical performance of NTC-epoxy composite thermistors,"As demand rises for flexible electronics, traditionally prepared sintered ceramic sensors must be transformed into fully new sensor materials that can bend and flex in use and integration. Negative temperature coefficient of resistance (NTC) ceramic thermistors are preferred temperature sensors for their high accuracy and excellent stability, yet their high stiffness and high temperature fabrication process limits their use in flexible electronics. Here, a low stiffness thermistor based on NTC ceramic particles of micron size embedded in an epoxy polymer matrix is reported. The effect of particle-to-particle contact on electrical performance is studied by arranging the NTC particles in the composite films in one of three ways: 1) Low particle contact, 2) Improved particle contact perpendicular to the electrodes and 3) dispersing high particle contact agglomerated clumps throughout the polymer. At 50 vol.\% of agglomerated NTC particles, the composite films exhibit a $\beta$-value of 2069 K and a resistivity, $\rho$, of 3.3$\cdot 10^5$ $\Omega$m, 4 orders of magnitude lower than a randomly dispersed composite at identical volume. A quantitative analysis shows that attaining a predominantly parallel connectivity of the NTC particles and polymer is a key parameter in determining the electrical performance of the composite film.",1911.07468v2 2021-03-11,Review on quasi-2D square planar nickelates,"In strongly correlated materials, lattice, charge, spin and orbital degrees of freedom interact with each other, leading to emergent physical properties such as superconductivity, colossal magnetic resistance and metal-insulator transition. Quasi-2D square planar nickelates, Rn+1NinO2n+2 (R=rare earth, n=2, 3...), are of significant interest and long sought for cuprate analogue due to the 3d9 electronic configuration of Ni+, the same as the active ion Cu2+ in the high-Tc superconducting cuprates. The field has attracted intense attention since 2019 due to the discovery of superconductivity in thin films of Nd0.8Sr0.2NiO2, although no superconductivity has been reported in bulk polycrystalline powders. Herein, we review the synthesis of polycrystalline powders of quasi-2D square planar nickelates through topotactic reduction of parent compounds that are synthesized via solid state reaction, precursor method, high pressure floating zone method and high-pressure flux method. We emphasize single crystal preparation using the high-pressure floating zone techniques. We discuss their crystal structure and physical properties including resistivity, magnetic susceptibility and heat capacity. We highlight the cuprate-like physics, including charge/spin stripes and large orbital polarization, identified in single crystals of R4Ni3O8 (R=La and Pr) combining synchrotron X-ray/neutron single crystal diffraction and density functional theory calculations. Furthermore, the challenges and possible research directions of this fast-moving field in the future are briefly discussed.",2103.06674v1 2022-05-25,Stranger than Metals,"Although the resistivity in traditional metals increases with temperature, its $T$ dependence vanishes at low or high temperature, albeit for different reasons. Here, we review a class of materials, known as \lq strange' metals, that can violate both principles. In materials exhibiting such behavior, the change in slope of the resistivity as the mean free path drops below the lattice constant, or as $T \rightarrow 0$, can be imperceptible, suggesting complete continuity between the charge carriers at low and high $T$. Since particles cannot scatter at length scales shorter than the interatomic spacing, strange metallicity calls into question the relevance of locality and a particle picture of the underlying current. This review focuses on transport and spectroscopic data on candidate strange metals with an eye to isolate and identify a unifying physical principle. Special attention is paid to quantum criticality, Planckian dissipation, Mottness, and whether a new gauge principle, which has a clear experimental signature, is needed to account for the non-local transport seen in strange metals. For the cuprates, strange metallicity is shown to track the superfluid density, thereby making a theory of this state the primary hurdle in solving the riddle of high-temperature superconductivity.",2205.12979v1 2024-03-08,Experimental set-up for thermal measurements at the nanoscale using an SThM probe with niobium nitride thermometer,"Scanning Thermal Microscopy (SThM) has become an important measurement tool for characterizing the thermal properties of materials at the nanometer scale. This technique requires a SThM probe that combines an Atomic Force Microscopy (AFM) probe and a very sensitive resistive thermometry; the thermometer being located at the apex of the probe tip allows the mapping of temperature or thermal properties of nanostructured materials with very high spatial resolution. The high interest of the SThM technique in the field of thermal nanoscience currently suffers from a low temperature sensitivity despite its high spatial resolution. To address this challenge, we developed a high vacuum-based AFM system hosting a highly sensitive niobium nitride (NbN) SThM probe to demonstrate its unique performance. As a proof of concept, we utilized this custom-built system to carry out thermal measurements using the 3$\omega$ method. By measuring the $V_{3\omega}$ voltage on the NbN resistive thermometer in vacuum conditions we were able to determine the SThM probe's thermal conductance and thermal time constant. The performance of the probe is demonstrated by doing thermal measurements in-contact with a sapphire sample.",2403.05405v2 2015-12-17,A Novel Material for In Situ Construction on Mars: Experiments and Numerical Simulations,"A significant step in space exploration during the 21st century will be human settlement on Mars. Instead of transporting all the construction materials from Earth to the red planet with incredibly high cost, using Martian soil to construct a site on Mars is a superior choice. Knowing that Mars has long been considered a ""sulfur-rich planet"", a new construction material composed of simulated Martian soil and molten sulfur is developed. In addition to the raw material availability for producing sulfur concrete and a strength reaching similar or higher levels of conventional cementitious concrete, fast curing, low temperature sustainability, acid and salt environment resistance, 100% recyclability are appealing superior characteristics of the developed Martian Concrete. In this study, different percentages of sulfur are investigated to obtain the optimal mixing proportions. Three point bending, unconfined compression and splitting tests were conducted to determine strength development, strength variability, and failure mechanisms. The test results show that the strength of Martian Concrete doubles that of sulfur concrete utilizing regular sand. It is also shown that the particle size distribution plays an important role in the mixture's final strength. Furthermore, since Martian soil is metal rich, sulfates and, potentially, polysulfates are also formed during high temperature mixing, which might contribute to the high strength. The optimal mix developed as Martian Concrete has an unconfined compressive strength of above 50 MPa. The formulated Martian Concrete is simulated by the Lattice Discrete Particle Model (LDPM), which exhibits excellent ability in modeling the material response under various loading conditions.",1512.05461v3 1998-09-07,Metallic temperature dependence of resistivity in perchlorate doped polyacetylene,"We have measured the electrical resistivity ($\rho$) and the thermoelectric power (TEP) of the perchlorate (ClO4^-) doped stretch oriented polyacetylene (PA) film. For the highly conducting samples ($\sigma_{RT} > 41000 S/cm$), the temperature dependence of the 4-probe resistivity shows positive temperature coefficient of resistivity (TCR) from T=1.5K to 300K. For the less conducting samples, the 4-probe resistivity data show the crossover of TCR with a broad minimum peak at T=T* > 200K. For samples of $\sigma_{RT}$$>$20000 S/cm, the $\rho (1.5K)/\rho (300K) <1$, i.e., the resistivity at 1.5K is lower than the room temperature resistivity value. The temperature dependence of the TEP shows diffusive linear metallic TEP becoming temperature independent below 40K. Unlike the others who used Cu(ClO_4)_2 for the ClO_4^- doping, the initial doping material we used is anhydrous Fe(ClO_4)_3 which is crucial to obtain the positive TCR from T=1.5K to 300K.",9809106v1 2006-11-20,Using Cluster Dynamics to Model Electrical Resistivity Measurements in Precipitating Al-Sc Alloys,"Electrical resistivity evolution during precipitation in Al-Sc alloys is modeled using cluster dynamics. This mesoscopic modeling has already been shown to correctly predict the time evolution of the precipitate size distribution. In this work, we show that it leads too to resistivity predictions in quantitative agreement with experimental data. We only assume that all clusters contribute to the resistivity and that each cluster contribution is proportional to its area. One interesting result is that the resistivity excess observed during coarsening mainly arises from large clusters and not really from the solid solution. As a consequence, one cannot assume that resistivity asymptotic behavior obeys a simple power law as predicted by LSW theory for the solid solution supersaturation. This forbids any derivation of the precipitate interface free energy or of the solute diffusion coefficient from resistivity experimental data in a phase-separating system like Al-Sc supersaturated alloys.",0611524v1 2008-10-06,Strong resistance nonlinearity and third harmonic generation in the unipolar resistance switching of NiO thin films,"We investigated third harmonic generation in NiO thin films, which exhibit unipolar resistance switching behavior. We found that the low resistance states of the films were strongly nonlinear, with variations in the resistance R as large as 60%. This strong nonlinear behavior was most likely caused by Joule heating of conducting filaments inside the films. By carefully controlling the applied dc bias, we obtained several low resistance states, whose values of the third harmonic coefficient B3f were proportional to R2+w (with w = 2.07). This suggested that the resistance changes of the NiO films were accompanied by connectivity changes of the conducting filaments, as observed in classical percolating systems.",0810.0886v1 2009-07-19,Current Driven tri-stable Resistance States in Magnetic Point Contacts,"Point contacts between normal and ferromagnetic metals are investigated using magneto-resistance and transport spectroscopy measurements combined with micromagnetic simulations. Pronounced hysteresis in the point-contact resistance versus both bias current and external magnetic field are observed. It is found that such hysteretic resistance can exhibit, in addition to bi-stable resistance states found in ordinary spin valves, tri-stable resistance states with a middle resistance level. We interpret these observation in terms of surface spin-valve and spin-vortex states, originating from a substantially modified spin structure at the ferromagnetic interface in contact core. We argue that these surface spin states, subject to a weakened exchange interaction, dominate the effects of spin transfer torques on the nanometer scale.",0907.3286v1 2014-03-25,Electric-Field-Modulated Nonvolatile Resistance Switching in VO2/PMN-PT(111) Heterostructures,"The electric-field-modulated resistance switching in VO2 thin films grown on piezoelectric (111)-0.68Pb(Mg1/3Nb2/3)O3-0.32PbTiO3 (PMN-PT) substrates has been investigated. Large relative change in resistance (10.7%) was observed in VO2/PMN-PT(111) hererostructures at room temperature. For a substrate with a given polarization direction, stable resistive states of VO2 films can be realized even when the applied electric fields are removed from the heterostructures. By sweeping electric fields across the heterostructure appropriately, multiple resistive states can be achieved. These stable resistive states result from the different stable remnant strain states of substrate, which is related to the rearrangements of ferroelectric domain structures in PMN-PT(111) substrate. The resistance switching tuned by electric field in our work may have potential applications for novel electronic devices.",1403.6388v2 2015-02-23,Phonon residual resistance of pure crystals,"Using the Boltzmann transport equation, we study phonon residual resistance of perfect metallic crystals of a finite thickness $d$ along which a weak constant electric field $E$ is applied. This resistance which is $\propto d^{-5}E^{-3}$, is due to scattering of electric field-heated electrons with emission of long-wave acoustic phonons. This electron-phonon interaction is caused by zero-point vibrations of the atoms in the perfect crystal lattice sites. Consideration is carried out for Cu, Ag and Au single crystals with the thickness of about 1 cm, in the fields of the order of 1 mV/cm. Following the Matthiessen rule, the resistance of the pure crystals the thicknesses of which are much larger than the electron mean free path, is represented as the sum of the impurity and phonon residual resistances. The condition on the thickness $d$ and the field $E$ is found at which the phonon scattering of the field-heated electrons dominates. Under this condition, the low-temperature resistances of pure crystals do not depend on the their purity and determine the phonon residual resistivity of the ideal crystals. The calculations are performed for Cu with a purity of at least 99.9999%.",1502.06486v2 2016-02-25,"Electric fields, weighting fields, signals and charge diffusion in detectors including resistive materials","In this report we discuss static and time dependent electric fields in detector geometries with an arbitrary number of parallel layers of a given permittivity and weak conductivity. We derive the Green's functions i.e. the field of a point charge, as well as the weighting fields for readout pads and readout strips in these geometries. The effect of 'bulk' resistivity on electric fields and signals is investigated. The spreading of charge on thin resistive layers is also discussed in detail, and the conditions for allowing the effect to be described by the diffusion equation is discussed. We apply the results to derive fields and induced signals in Resistive Plate Chambers, Micromega detectors including resistive layers for charge spreading and discharge protection as well as detectors using resistive charge division readout like the MicroCAT detector. We also discuss in detail how resistive layers affect signal shapes and increase crosstalk between readout electrodes.",1602.07949v1 2016-02-26,Investigating the Temperature Effects on Resistive Random Access Memory (RRAM) Devices,"In this paper, we report the effect of filament radius and filament resistivity on the saturated temperature of ZnO, TiO2, WO3 and HfO2 Resistive Random Access Memory (RRAM) devices. We resort to the thermal reaction model of RRAM for the present analysis. The results substantiate decrease in saturated temperature with increase in the radius and resistivity of filament for the investigated RRAM devices. Moreover, a sudden change in the saturated temperature at a lower value of filament radius and resistivity is observed as against the steady change at the medium and higher value of the filament radius and resistivity. Results confirm the dependence of saturated temperature on the filament size and resistivity in RRAM.",1602.08262v1 2017-11-02,Resistivity scaling model for metals with conduction band anisotropy,"It is generally understood that the resistivity of metal thin films scales with film thickness mainly due to grain boundary and boundary surface scattering. Recently, several experiments and ab initio simulations have demonstrated the impact of crystal orientation on resistivity scaling. The crystal orientation cannot be captured by the commonly used resistivity scaling models and a qualitative understanding of its impact is currently lacking. In this work, we derive a resistivity scaling model that captures grain boundary and boundary surface scattering as well as the anisotropy of the band structure. The model is applied to Cu and Ru thin films, whose conduction bands are (quasi-)isotropic and anisotropic respectively. After calibrating the anisotropy with ab initio simulations, the resistivity scaling models are compared to experimental resistivity data and a renormalization of the fitted grain boundary reflection coefficient can be identified for textured Ru.",1711.00796v3 2021-02-05,Does Non-Genetic Heterogeneity Facilitate the Development of Genetic Drug Resistance?,"Non-genetic forms of antimicrobial drug resistance can result from cell-to-cell variability that is not encoded in the genetic material. Data from recent studies also suggest that non-genetic mechanisms can facilitate the development of genetic drug resistance. In this Perspective article, we speculate on how the interplay between non-genetic and genetic mechanisms may affect microbial adaptation and evolution during drug treatment. We argue that cellular heterogeneity arising from fluctuations in gene expression, epigenetic modifications, as well as genetic changes contributes to drug resistance at different timescales, and that the interplay between these mechanisms may influence the evolutionary dynamics of pathogen resistance. Accordingly, developing a better understanding of non-genetic mechanisms in drug resistance and how they interact with genetic mechanisms will enhance our ability to combat antimicrobial resistance.",2102.03276v1 2023-04-10,T-square dependence of the electronic thermal resistivity in metallic strontium titanate,"The temperature dependence of the phase space for electron-electron (e-e) collisions leads to a T-square contribution to electrical resistivity of metals. Umklapp scattering are identified as the origin of momentum loss due to e-e scattering in dense metals. However, in dilute metals like lightly doped strontium titanate, the origin of T-square electrical resistivity in absence of Umklapp events is yet to be pinned down. Here, by separating electron and phonon contributions to heat transport, we extract the electronic thermal resistivity in niobium-doped strontium titanate and show that it also displays a T-square temperature dependence. Its amplitude correlates with the T-square electrical resistivity. The Wiedemann-Franz law strictly holds in the zero-temperature limit, but not at finite-temperature, because the two T-square prefactors are different by a factor of $\approx 3$, like in other Fermi liquids. Recalling the case of $^3$He, we argue that T-square thermal resistivity does not require Umklapp events. The approximate recovery of the Wiedemann-Franz law in presence of disorder would account for a T-square electrical resistivity without Umklapp.",2304.04841v2 2001-07-03,Low temperature resistance minimum in non-superconducting 3R-Nb_{1+x}S_2 and 3R-Ga_xNbS_2,"We report the structural and electron transport properties of 3R-Nb_{1+x}S_2 (x >= .07) and 3R-Ga_xNbS_2 (.1 <= x <= .33) prepared as polycrystalline pellets as well as single crystals grown by vapour transport. We observe a resistance minimum in these compounds between 20-60 K, with the T_min proportional to x. The resistance scales as rho/rho_min(T/T_min) between .2 < T/T_min < 2 for different phases with x <= .25 whose resistivity differs by an order of magnitude. Powder X-ray diffraction (XRD) also shows progressively increasing intensity of superlattice lines with cation concentration. The thermopower changes sign around the resistance minimum. The explanation of the resistance minimum and the simultaneous rapid suppression of superconductivity is sought in e-e scattering effects in the presence of cation disorder in these narrow band anisotropic materials.",0107067v1 2006-08-11,Fracture resistance via topology optimisation,"The fracture resistance of structures is optimised using the level-set method. Fracture resistance is assumed to be related to the elastic energy released by a crack propagating in a normal direction from parts of the boundary which are in tension, and is calculated using the virtual crack extension technique. The shape derivative of the fracture-resistance objective function is derived. Two illustrative two-dimensional case studies are presented: a hole in a plate subjected to biaxial strain; and a bridge fixed at both ends subjected to a single load in which the compliance and fracture resistance are jointly optimised. The structures obtained have rounded corners and more material at places where they are in tension. Based on the results, we propose that fracture resistance may be modelled more easily but less directly by including a term proportional to surface area in the objective function, in conjunction with non-linear elasticity where the Young's modulus in tension is lower than in compression.",0608260v1 2016-05-19,Resistive Switching Phenomena of HfO2 Films Grown by MOCVD for Resistive Switching Memory Devices,"The resistive switching phenomena of HfO2 films grown by metalorganic chemical vapor deposition was studied for the application of ReRAM devices. In the fabricated Pt/HfO2/TiN memory cells, the bipolar resistive switching characteristics were observed, and the set and reset states were measured to be as low as 7 uA and 4 uA, respectively, at VREAD = 1 V. Regarding the resistive switching performance, the stable RS performance was observed under 40 repetitive dc cycling test with the small variations of set/reset voltages and currents, and good retention characteristics over 105 s in both LRS and HRS. These results show the possibility of MOCVD grown HfO2 films as a promising resistive switching materials for ReRAM applications.",1605.06014v1 2020-02-10,Resistivity minimum in diluted metallic magnets,"Resistivity minima are commonly seen in itinerant magnets and they are often attributed to the Kondo effect. However, recent experiments are revealing an increasing number of materials showing resistivity minima in the absence of indications of Kondo singlet formation. In a previous work [Z. Wang, K. Barros, G.-W. Chern, D. L. Maslov, and C. D. Batista, Phys. Rev. Lett. 117, 206601 (2016)], we demonstrated that the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction can produce a classical spin liquid state at finite temperature, whose resistivity increases with decreasing temperature. The classical spin liquid exists over a relatively large temperature window because of the frustrated nature of the RKKY interaction produced by a 2D electron gas. In this work, we investigate the robustness of the RKKY-induced resistivity upturn against site dilution, which provides an alternative, and more robust, way of stabilizing the classical spin liquid state down to T=0. By using series expansions and stochastic Landau-Lifshitz dynamics simulation, we show that site dilution competes with thermal fluctuations and further stabilizes the resistivity upturn, which is accompanied by a negative magnetoresistivity due to suppression of the electron-spin scattering.",2002.03858v2 2021-10-06,Pinpointing the Dominant Component of Contact Resistance to Atomically Thin Semiconductors,"Achieving good electrical contacts is one of the major challenges in realizing devices based on atomically thin two-dimensional (2D) semiconductors. Several studies have examined this hurdle, but a universal understanding of the contact resistance and an underlying approach to its reduction are currently lacking. In this work we expose the shortcomings of the classical contact resistance model in describing contacts to 2D materials, and offer a correction based on the addition of a lateral pseudo-junction resistance component (Rjun). We use a combination of unique contact resistance measurements to experimentally characterize Rjun for Ni contacts to monolayer MoS2. We find that Rjun is the dominating component of the contact resistance in undoped 2D devices and show that it is responsible for most of the back-gate bias and temperature dependence. Our corrected model and experimental results help understand the underlying physics of state-of-the-art contact engineering approaches in the context of minimizing Rjun.",2110.02563v1 2023-11-14,Giant Resistance Switch in Twisted Transition Metal Dichalcogenide Tunnel Junctions,"Resistance switching in multilayer structures are typically based on materials possessing ferroic orders. Here we predict an extremely large resistance switching based on the relative spin-orbit splitting in twisted transition metal dichalcogenide (TMD) monolayers tunnel junctions. Because of the valence band spin splitting which depends on the valley index in the Brillouin zone, the perpendicular electronic transport through the junction depends on the relative reciprocal space overlap of the spin-dependent Fermi surfaces of both layers, which can be tuned by twisting one layer. Our quantum transport calculations reveal a switching resistance of up to $10^6 \%$ when the relative alignment of TMDs goes from $0^{\circ}$ to $60^{\circ}$ and when the angle is kept fixed at $60^{\circ}$ and the Fermi level is varied. By creating vacancies, we evaluate how inter-valley scattering affects the efficiency and find that the resistance switching remains large ($10^4 \%$) for typical values of vacancy concentration. Not only this resistance switching should be observed at room temperature due to the large spin splitting, but our results show how twist angle engineering and control of van der Waals heterostructures could be used for next-generation memory and electronic applications.",2311.08397v1 2000-10-24,Slater Transition in the Pyrochlore Cd2Os2O7,"Cd2Os2O7 crystallizes in the pyrochlore structure and undergoes a metal-insulator transition (MIT) near 226 K. We have characterized the MIT in Cd2Os2O7 using X-ray diffraction, resistivity at ambient and high pressure, specific heat, magnetization, thermopower, Hall coefficient, and thermal conductivity. Both single crystals and polycrystalline material were examined. The MIT is accompanied by no change in crystal symmetry and a change in unit cell volume of less than 0.05%. The resistivity shows little temperature dependence above 226 K, but increases by 3 orders of magnitude as the sample is cooled to 4 K. The specific heat anomaly resembles a mean-field transition and shows no hysteresis or latent heat. Cd2Os2O7 orders magnetically at the MIT. The magnetization data is consistent with antiferromagnetic order, with a small parasitic ferromagnetic component. The Hall and Seebeck coefficients are consistent with a semiconducting gap opening at the Fermi energy at the MIT. We have also performed electronic structure calculations on Cd2Os2O7. These calculations indicate that Cd2Os2O7 is metallic, with a sharp peak in the density of states at the Fermi energy. We intepret the data in terms of a Slater transition. In this scenario, the MIT is produced by a doubling of the unit cell due to the establishment of antiferromagnetic order. A Slater transition-unlike a Mott transition-is predicted to be continuous, with a semiconducting energy gap opening much like a BCS gap as the material is cooled below $T_{MIT}$.",0010364v1 2004-12-17,Origin of Colossal Dielectric Response of Pr(0.6)Ca(0.4)MnO(3),"We report the detailed study of dielectric response of Pr(0.6)Ca(0.4)MnO(3) (PCMO), member of manganite family showing colossal magnetoresistance. Measurements have been performed on four polycrystalline samples and four single crystals, allowing us to compare and extract the essence of dielectric response in the material. High frequency dielectric function is found to be 30, as expected for the perovskite material. Dielectric relaxation is found in frequency window of 20Hz-1MHz at temperatures of 50-200K that yields to colossal low-frequency dielectric function, i.e. static dielectric constant. Static dielectric constant is always colossal, but varies considerably in different samples from 1000 until 100000. The measured data can be simulated very well by blocking (surface barrier) capacitance in series with sample resistance. This indicates that the large dielectric constant in PCMO arises from the Schottky barriers at electrical contacts. Measurements in magnetic field and with d.c. bias support this interpretation. Weak anomaly at the charge ordering temperature can also be attributed to interplay of sample and contact resistance. We comment our results in the framework of related studies by other groups.",0412473v3 2012-05-14,Bi2Te1.6S1.4 - a Topological Insulator in the Tetradymite Family,"We describe the crystal growth, crystal structure, and basic electrical properties of Bi2Te1.6S1.4, which incorporates both S and Te in its Tetradymite quintuple layers in the motif -[Te0.8S0.2]-Bi-S-Bi-[Te0.8S0.2]-. This material differs from other Tetradymites studied as topological insulators due to the increased ionic character that arises from its significant S content. Bi2Te1.6S1.4 forms high quality crystals from the melt and is the S-rich limit of the ternary Bi-Te-S {\gamma}-Tetradymite phase at the melting point. The native material is n-type with a low resistivity; Sb substitution, with adjustment of the Te to S ratio, results in a crossover to p-type and resistive behavior at low temperatures. Angle resolved photoemission study shows that topological surface states are present, with the Dirac point more exposed than it is in Bi2Te3 and similar to that seen in Bi2Te2Se. Single crystal structure determination indicates that the S in the outer chalcogen layers is closer to the Bi than the Te, and therefore that the layers supporting the surface states are corrugated on the atomic scale.",1205.2924v1 2015-05-26,"Transport, Magnetic and Vibrational Properties of Chemically Exfoliated Few Layer Graphene","We study the vibrational, magnetic and transport properties of Few Layer Graphene (FLG) using Raman and electron spin resonance spectroscopy and microwave conductivity measurements. FLG samples were produced using wet chemical exfoliation with different post-processing, namely ultrasound treatment, shear mixing, and magnetic stirring. Raman spectroscopy shows a low intensity D mode which attests a high sample quality. The G mode is present at $1580$ cm$^{-1}$ as expected for graphene. The 2D mode consists of 2 components with varying intensities among the different samples. This is assigned to the presence of single and few layer graphene in the samples. ESR spectroscopy shows a main line in all types of materials with a width of about $1$ mT and and a $g$-factor in the range of $2.005-2.010$. Paramagnetic defect centers with a uniaxial $g$-factor anisotropy are identified, which shows that these are related to the local sp$^2$ bonds of the material. All kinds of investigated FLGs have a temperature dependent resistance which is compatible with a small gap semiconductor. The difference in resistance is related to the different grain size of the samples.",1505.06857v1 2017-02-10,Highly wear-resistant and low-friction Si3N4 composites by addition of graphene nanoplatelets approaching the 2D limit,"Graphene nanoplatelets (GNPs) have emerged as one of the most promising filler materials for improving the tribological performance of ceramic composites due to their outstanding solid lubricant properties as well as mechanical and thermal stability. Yet, the addition of GNPs has so far provided only a very limited improvement in the tribological properties of ceramics, particularly concerning the reduction of their friction coefficient. This is most likely due to the challenges of achieving a lubricating and protecting tribo-film through a high GNP coverage of the exposed surfaces. Here we show that this can be achieved by efficiently increasing the exfoliation degree of GNPs down to the few-layer (FL) range. By employing FL-GNPs as filler material, the wear resistance of Si3N4 composites can be increased by about twenty times, the friction coefficient reduced to nearly its half, while the other mechanical properties are also preserved or improved. Using confocal Raman microscopy, we were able to demonstrate the formation of a continuous FL- GNP tribo-film, already at 5wt% FL-GNP content.",1702.03153v1 2017-12-16,Stress-dependent electrical transport and its universal scaling in granular materials,"We experimentally and numerically examine stress-dependent electrical transport in granular materials to elucidate the origins of their universal dielectric response. The ac responses of granular systems under varied compressive loadings consistently exhibit a transition from a resistive plateau at low frequencies to a state of nearly constant loss at high frequencies. By using characteristic frequencies corresponding to the onset of conductance dispersion and measured direct-current resistance as scaling parameters to normalize the measured impedance, results of the spectra under different stress states collapse onto a single master curve, revealing well-defined stress-independent universality. In order to model this electrical transport, a contact network is constructed on the basis of prescribed packing structures, which is then used to establish a resistor-capacitor network by considering interactions between individual particles. In this model the frequency-dependent network response meaningfully reproduces the experimentally observed master curve exhibited by granular materials under various normal stress levels indicating this universal scaling behaviour is found to be governed by i) interfacial properties between grains and ii) the network configuration. The findings suggest the necessity of considering contact morphologies and packing structures in modelling electrical responses using network-based approaches.",1712.05938v2 2020-04-06,Spin Hall magnetoresistance in antiferromagnetic insulators,"Antiferromagnetic materials promise improved performance for spintronic applications, as they are robust against external magnetic field perturbations and allow for faster magnetization dynamics compared to ferromagnets. The direct observation of the antiferromagnetic state, however, is challenging due to the absence of a macroscopic magnetization. Here, we show that the spin Hall magnetoresistance (SMR) is a versatile tool to probe the antiferromagnetic spin structure via simple electrical transport experiments by investigating the easy-plane antiferromagnetic insulators $\alpha$-Fe2O3 (hematite) and NiO in bilayer heterostructures with a Pt heavy metal top electrode. While rotating an external magnetic field in three orthogonal planes, we record the longitudinal and the transverse resistivities of Pt and observe characteristic resistivity modulations consistent with the SMR effect. We analyze both their amplitude and phase and compare the data to the results from a prototypical collinear ferrimagnetic Y3Fe5O12/Pt bilayer. The observed magnetic field dependence is explained in a comprehensive model, based on two magnetic sublattices and taking into account magnetic field-induced modifications of the domain structure. Our results show that the SMR allows us to understand the spin configuration and to investigate magnetoelastic effects in antiferromagnetic multi-domain materials. Furthermore, in $\alpha$-Fe2O3/Pt bilayers, we find an unexpectedly large SMR amplitude of $2.5 \times 10^{-3}$, twice as high as for prototype Y3Fe5O12/Pt bilayers, making the system particularly interesting for room-temperature antiferromagnetic spintronic applications.",2004.02639v2 2017-04-11,Transfer of Vertical Graphene Nanosheets onto Flexible Substrates towards Supercapacitor Application,"Vertical graphene nanosheets (VGNs) are the material of choice for next-generation electronic device applications. The growing demand for flexible devices in electronic industry brings in restriction on growth temperature of the material of interest. However, VGNs with better structural quality is usually achieved at high growth temperatures. The difficulty associated with the direct growth on flexible substrates can overcome by adopting an effective strategy of transferring the well grown VGNs onto arbitrary flexible substrates through soft chemistry route. Hence, we demonstrated a simple, inexpensive and scalable technique for the transfer of VGNs onto arbitrary substrates without disrupting its morphology and structural properties. After transfer, the morphology, chemical structure and electronic properties are analyzed by scanning electron microscopy, Raman spectroscopy and four probe resistive methods, respectively. Associated characterization investigation indicates the retention of morphological, structural and electrical properties of transferred VGNs compared to as-grown one. Furthermore the storage capacity of the VGNs transferred onto flexible substrates is also examined. A very lower sheet resistance of 0.67 kOhm/sq. and excellent supercapacitance of 158 micro-Farrad/cm2 with 91.4% retention after 2000 cycles confirms the great prospective of this damage-free transfer approach of VGNs for flexible nanoelectronic device applications",1704.03227v1 2019-03-26,Isostructural Mott Transition in 2D honeycomb antiferromagnet V$_{0.9}$PS$_3$,"We present the observation of an isostructural Mott insulator-metal transition in van-der-Waals honeycomb antiferromagnet V$_{0.9}$PS$_3$ through high-pressure x-ray diffraction and transport measurements. The MPX$_3$ family of magnetic van-der-Waals materials (M denotes a first row transition metal and X either S or Se) are currently the subject of broad and intense attention, but the vanadium compounds have until this point not been studied beyond their basic properties. We observe insulating variable-range-hopping type resistivity in V$_{0.9}$PS$_3$, with a gradual increase in effective dimensionality with increasing pressure, followed by a transition to a metallic resistivity temperature dependence between 112 and 124 kbar. The metallic state additionally shows a low-temperature upturn we tentatively attribute to the Kondo Effect. A gradual structural distortion is seen between 26-80 kbar, but no structural change at higher pressures corresponding to the insulator-metal transition. We conclude that the insulator-metal transition occurs in the absence of any distortions to the lattice - an isostructural Mott transition in a new class of two-dimensional material, and in strong contrast to the behavior of the other MPX$_3$ compounds.",1903.10971v1 2019-03-29,Substrate Mediated Synthesis of Ti-Si-N Nano-and-Micro Structures for Optoelectronic Applications,"Being one of the strongest materials, ternary TiSiN exhibits a very interesting family of binary transition metal nitride and silicide systems. A novel technique to fabricate morphologically fascinating nano and micro structures of TiSiN is reported here. The referred TiSiN films, majorly constituted with cubic TiN phase, are enriched with crystalline nanoparticles, micro-flowers and faceted micro-crystals which possess attractive functionalities towards plasmon mediated optoelectronic applications. Reactivity of titanium to silicon nitride based dielectric topping on the substrate at high temperature plays the key role in nitride formation for the demonstrated protocol. The optoelectronic response for these morphologically enriched composite films indicates an influential role of photo-induced surface plasmon polaritons on their dc transport properties. A plasmonically tuned resistive switching, controlled by the surface morphology in association with the film thickness, is observed under light illumination. Using Drudes modified frequency dependent bulk electron scattering rates and surface mediated SPPs-electron scattering rates, a generic model is proposed for addressing unambiguously the increased device resistance in response to light. The featured synthesis process opens a new direction towards the growth of transition metal nitrides while the proposed model serves as a basic platform to understand photo-induced electron scattering mechanisms in metal.",1903.12376v1 2020-01-06,Controlled introduction of defects to delafossite metals by electron irradiation,"The delafossite metals PdCoO$_{2}$, PtCoO$_{2}$ and PdCrO$_{2}$ are among the highest conductivity materials known, with low temperature mean free paths of tens of microns in the best as-grown single crystals. A key question is whether these very low resistive scattering rates result from strongly suppressed backscattering due to special features of the electronic structure, or are a consequence of highly unusual levels of crystalline perfection. We report the results of experiments in which high energy electron irradiation was used to introduce point disorder to the Pd and Pt layers in which the conduction occurs. We obtain the cross-section for formation of Frenkel pairs in absolute units, and cross-check our analysis with first principles calculations of the relevant atomic displacement energies. We observe an increase of resistivity that is linear in defect density with a slope consistent with scattering in the unitary limit. Our results enable us to deduce that the as-grown crystals contain extremely low levels of in-plane defects of approximately $0.001\%$. This confirms that crystalline perfection is the most important factor in realizing the long mean free paths, and highlights how unusual these delafossite metals are in comparison with the vast majority of other multi-component oxides and alloys. We discuss the implications of our findings for future materials research.",2001.01471v1 2020-01-17,Wettability and surface energy of parylene F,"Parylenes are barrier materials employed as protective layers. However, many parylenes are unsuitable for applications under harsh conditions. A new material, parylene F, demonstrates considerable potential for a wide range of applications due to its high temperature and UV resistance. For the first time, the wettability and surface energy of parylene F were investigated to determine the feasibility of parylene F as an alternative to the commonly employed parylene C. The results show that parylene F has a hydrophobic surface with a water contact angle of 109.63 degrees. We found that 3.5 ul probe liquid is an optimal value for the contact angle measurement of parylene F. Moreover, we found that the Owens-Wendt-Kaelble and the Lifshitz-van der Waals/acid-base approaches are unsuitable for determining the surface energy of parylene F, whereas an approach based on the limitless liquid-solid interface wetting system is compatible. Furthermore, the results show that parylene F has a surface energy of 39.05 mJ/m2. Considering the improved resistance, relatively low cost, and the desirable properties, parylene F can replace parylene C for applications under harsh conditions.",2001.06146v2 2020-01-24,Adaptive hard and tough mechanical response in single-crystal B1 VNx ceramics via control of anion vacancies,"High hardness and toughness are generally considered mutually exclusive properties for single-crystal ceramics. Combining experiments and ab initio molecular dynamics (AIMD) atomistic simulations at room temperature, we demonstrate that both the hardness and toughness of single-crystal NaCl-structure VNx/MgO(001) thin films are simultaneously enhanced through the incorporation of anion vacancies. Nanoindentation results show that VN0.8, here considered as representative understoichiometric VNx system, is ~20% harder, as well as more resistant to fracture than stoichiometric VN samples. AIMD modeling of VN and VN0.8 supercells subjected to [001] and [110] elongation reveal that the tensile strengths of the two materials are similar. Nevertheless, while the stoichiometric VN phase systematically cleaves in a brittle manner at tensile yield points, the understoichiometric compound activates transformation-toughening mechanisms that dissipate accumulated stresses. AIMD simulations also show that VN0.8 exhibits an initially greater resistance to both {110}<1-10> and {111}<1-10> shear deformation than VN. However, for progressively increasing shear strains, the VN0.8 mechanical behavior gradually evolves from harder to more ductile than VN. The transition is mediated by anion vacancies, which facilitate {110}<1-10> and {111}<1-10> lattice slip by reducing activation shear stresses by as much as 35%. Electronic-structure analyses show that the two-regime hard/tough mechanical response of VN0.8 primarily stems from its intrinsic ability to transfer d electrons between 2nd-neighbor and 4th-neighbor (i.e., across vacancy sites) V-V metallic states. Our work offers a route for electronic-structure design of hard materials in which a plastic mechanical response is triggered with loading.",2001.08933v2 2020-05-14,Gate- and Light-Tunable Negative Differential Resistance with High Peak Current Density in 1T-TaS$_2$/2H-MoS$_2$ T-Junction,"Metal-based electronics is attractive for fast and radiation-hard electronic circuits and remains one of the longstanding goals for researchers. The emergence of 1T-TaS$_2$, a layered material exhibiting strong charge density wave (CDW) driven resistivity switching that can be controlled by an external stimulus such as electric field and optical pulses, has triggered a renewed interest in metal-electronics. Here we demonstrate a negative differential resistor (NDR) using electrically driven CDW phase transition in an asymmetrically designed T-junction made up of 1T-TaS$_2$/2H-MoS$_2$ van der Waals heterostructure. The principle of operation of the proposed device is governed by majority carrier transport and is distinct from usual NDR devices employing tunneling of carriers, thus avoids the bottleneck of weak tunneling efficiency in van der Waals heterojunctions. Consequently, we achieve a peak current density in excess of $10^5$ nA$\mu$m$^{-2}$, which is about two orders of magnitude higher than that obtained in typical layered material based NDR implementations. The peak current density can be effectively tuned by an external gate voltage as well as photo-gating. The device is robust against ambiance-induced degradation and the characteristics repeat in multiple measurements over a period of more than a month. The findings are attractive for the implementation of active metal-based functional circuits.",2005.07146v2 2021-05-23,"Substrate-Versatile Direct-Write Printing of Carbon Nanotube-Based Flexible Conductors, Circuits, and Sensors","Printed electronics rely on the deposition of conductive liquid inks, typically onto polymeric or paper substrates. Among available conductive fillers for use in electronic inks, carbon nanotubes (CNTs) have high conductivity, low density, processability at low temperatures, and intrinsic mechanical flexibility. However, the electrical conductivity of printed CNT structures has been limited by CNT quality and concentration, and by the need for nonconductive modifiers to make the ink stable and extrudable. This study introduces a polymer-free, printable aqueous CNT ink, and presents the relationships between printing resolution, ink rheology, and ink-substrate interactions. A model is constructed to predict printed feature sizes on impermeable substrates based on Wenzel wetting. Printed lines have conductivity up to 10,000 S/m. The lines are flexible, with < 5% change in DC resistance after 1,000 bending cycles, and <3% change in DC resistance with a bending radius down to 1 mm. Demonstrations focus on (i) conformality, via printing CNTs onto stickers that can be applied to curved surfaces, (ii) interactivity using a CNT-based button printed onto folded paper structure, and (iii) capacitive sensing of liquid wicking into the substrate itself. Facile integration of surface mount components on printed circuits is enabled by the intrinsic adhesion of the wet ink.",2105.10942v1 2021-10-05,Nanoscale devices with superconducting electrodes to locally channel current in 3D Weyl semimetals,"We report on the fabrication of nano-devices on the \hkl[-1 0 1] surface of a Weyl semimetal, a macroscopic crystal of TaAs, and low-temperature transport measurements. We can implement electron beam lithography by peeling off and transferring the resist for nanofabrication onto the irregular crystal. We fabricate the device electrodes with superconducting Niobium nitride (NbN) to control the current flow through the intended active area of the devices. Our device structure enables the reduction of the current jetting effect, and we demonstrate the negative magnetoresistance measurement as a function of angle. The high field magnetotransport show three distinct oscillation frequencies corresponding to the three bands at the Fermi level. Resistance measured in the low magnetic field shows the usual weak anti-localization dip near the zero-field -- a signature of a Weyl material. Our method of fabricating devices with superconducting electrodes provides a way to probe the electrical properties of macroscopic single crystals at the nanoscale. As we use conventional lithographic techniques for patterning, this method can be extended to a wide gamut of electrode materials and a large class of 3D quantum materials.",2110.01793v1 2021-11-29,Doped graphene/carbon black hybrid catalyst giving enhanced oxygen reduction reaction activity with high resistance to corrosion in proton exchange membrane fuel cells,"Nitrogen doping of the carbon is an important method to improve the performance and durability of catalysts for proton exchange membrane fuel cells by platinum-nitrogen and carbon-nitrogen bonds. This study shows that p-phenyl groups and graphitic N acting bridges linking platinum and the graphene/carbon black (the ratio graphene/carbon black=2/3) hybrid support materials achieved the average size of platinum nanoparticles with (4.88 +/- 1.79) nm. It improved the performance of the lower-temperature hydrogen fuel cell up to 0.934 W cm-2 at 0.60 V, which is 1.55 times greater than that of commercial Pt/C. Doping also enhanced the interaction between Pt and the support materials, and the resistance to corrosion, thus improving the durability of the low-temperature hydrogen fuel cell with a much lower decay of 10 mV at 0.80 A cm-2 after 30k cycles of an in-situ accelerated stress test of catalyst degradation than that of 92 mV in Pt/C, which achieves the target of Department of Energy (<30 mV). Meanwhile, Pt/NrEGO2-CB3 remains 78% of initial power density at 1.5 A cm-2 after 5k cycles of in-situ accelerated stress test of carbon corrosion, which is more stable than the power density of commercial Pt/C, keeping only 54% after accelerated stress test.",2111.14648v1 2022-03-22,Traps and transport resistance: the next frontier for stable state-of-the-art non-fullerene acceptor solar cells,"Stability is one of the most important challenges facing organic solar cells (OSC) on their path to commercialization. In the high-performance material system PM6:Y6 studied here, investigate degradation mechanisms of inverted photovoltaic devices. We have identified two distinct degradation pathways: one requires presence of both illumination and oxygen and features a short-circuit current reduction, the other one is induced thermally and marked by severe losses of open-circuit voltage and fill factor. We focus our investigation on the thermally accelerated degradation. Our findings show that bulk material properties and interfaces remain remarkably stable, however, aging-induced defect state formation in the active layer remains the primary cause of thermal degradation. The increased trap density leads to higher non-radiative recombination, which limits open-circuit voltage and lowers charge carrier mobility in the photoactive layer. Furthermore, we find the trap-induced transport resistance to be the major reason for the drop in fill factor. Our results suggest that device lifetimes could be significantly increased by marginally suppressing trap formation, leading to a bright future for OSC.",2203.11905v1 2022-07-05,Phonons behave like Electrons in the Thermal Hall Effect of the Cuprates,"The thermal Hall effect, which arises when heat flows transverse to an applied thermal gradient, has become an important observable in the study of quantum materials. Recent experiments found a large thermal Hall conductivity $\kappa_{xy}$ in many high-temperature cuprate superconductors, including deep inside the Mott insulator, but the underlying mechanism remains unknown. Here, we uncover a surprising linear temperature dependence for the inverse thermal Hall resistivity, $1/\rho_H=-\kappa_{xx}^2/\kappa_{xy}$, in the Mott insulating cuprates $\mathrm{La_2CuO_4}$ and $\mathrm{Sr_2CuO_2Cl_2}$. We also find this linear scaling in the pseudogap state of Nd-LSCO in the out-of-plane direction, highlighting the importance of phonons. On the electron-doped side, the linear inverse thermal Hall signal emerges in NCCO and PCCO at various dopings, including in the strange metal. Although such dependence arises in the simple Drude model for itinerant electrons, its origin is unclear in strongly correlated Mott insulating or pseudogap states. We perform a Boltzmann analysis for phonons that incorporates skew-scattering, and we are able to identify regimes where a linear $T$ inverse Hall resistivity appears. Finally, we suggest future experiments that would further our fundamental understanding of heat transport in the cuprates, and other quantum materials.",2207.02240v3 2022-08-28,Multiferroic Ti$_3$C$_2$T$_x$ MXene with Tunable Ferroelectric-controlled High Performance Resistive Memory Devices,"Multiferroic (MF) devices based on simultaneous ferroelectric and ferromagnetic phenomena are considered to be promising candidates for future bi-functional micro/nano-electronics. The multiferroic phenomena in two-dimensional materials is rarely reported in literature. We reported a simple approach to reveal frequency-dependent ferroelectricity and mutiferroicity in Ti$_3$C$_2$T$_x$ MXene film at room-temperature. To study the frequency and poling effect on ferroelectricity as well as multiferroicity, we performed electric polarization vs. electric field measurement at different external frequencies measured under zero and non-zero static magnetic fields. In order to further investigate this effect, the magneto-electric (ME) coupling was also performed to confirm the multiferroic nature of our synthesized Ti$_3$C$_2$T$_x$ MXene film. The ferroelectric hysteresis effect was attributed to the switching of electric domain walls under low frequencies that continue to respond to at much extent to the higher frequencies. The coupling between disordered electric dipoles with local spin moments could cause presence of strong magneto-electric coupling. Moreover, the bipolar resistive switching in trilayer memory devices also supports the ferroelectric behavior of HT- Ti$_3$C$_2$T$_x$ MXene film and showed uniform repeatability in switching behavior due to minimum dielectric loss inside ferroelectric HT-Ti$_3$C$_2$T$_x$ MXene along with improved on/off ratio in comparison to non-ferroelectric Ti$_3$C$_2$T$_x$ MXene. The unique multiferroic behavior along with ferroelectric-tuned memristor devices reported here at room temperature will help understand the intrinsic nature of 2D materials and will establish novel data storage devices.",2208.13128v1 2023-08-05,Graphene-based RRAM devices for neural computing,"Resistive random access memory (RRAM) is very well known for its potential application in in-memory and neural computing. However, they often have different types of device-to-device and cycle-to-cycle variability. This makes it harder to build highly accurate crossbar arrays.Traditional RRAM designs make use of various filament-based oxide materials for creating a channel which is sandwiched between two electrodes to form a two-terminal structure. They are often subjected to mechanical and electrical stress over repeated read-and-write cycles. The behavior of these devices often varies in practice across wafer arrays over these stress when fabricated. The use of emerging 2D materials is explored to improve electrical endurance, long retention In review time, high switching speed, and fewer power losses. This study provides an in-depth exploration of neuro-memristive computing and its potential applications, focusing specifically on the utilization of graphene and 2D materials in resistive random-access memory (RRAM) for neural computing. The paper presents a comprehensive analysis of the structural and design aspects of graphene-based RRAM, along with a thorough examination of commercially available RRAM models and their fabrication techniques. Furthermore, the study investigates the diverse range of applications that can benefit from graphene-based RRAM devices.",2308.02767v1 2023-08-06,Mechanically exfoliated low-layered [Ca$_2$CoO$_3$]$_{0.62}$[CoO$_2$]: A single-crystalline p-type transparent conducting oxide,"Transparent conducting oxides (TCOs) are essential components of optoelectronic devices and various materials have been explored for highly efficient TCOs having a combination of high transmittance and low sheet resistance. Here, we focus on a misfit thermoelectric oxide [Ca$_2$CoO$_3$]$_{0.62}$[CoO$_2$] and fabricate the transparent low-layered crystals by a mechanical tape-peeling method using the single-crystalline samples. From the transmittance measurement, we find that the thickness of low-layered samples is several orders of hundred nanometers, which is comparable with the estimation from the scanning electron microscopy images. Compared to the previous results on the polycrystalline and $c$-axis oriented transparent films, the electrical resistivity is reduced owing to the single-crystalline nature. The figure of merit for the transparent conducting materials in the present low-layered samples is then evaluated to be higher than the values in the previous reports. The present results on the low-layered single-crystalline [Ca$_2$CoO$_3$]$_{0.62}$[CoO$_2$] may offer a unique class of multi-functional transparent thermoelectric oxides.",2308.03221v1 2023-09-06,Robust Sandwiched B/TM/B Structures by Metal Intercalating into Bilayer Borophene Leading to Excellent Hydrogen Evolution Reaction,"Bilayer borophene, very recently synthesized on Ag and Cu, possesses extremely flat large surface and excellent conductivity. Besides, the van der Waals gap of bilayer borophene can be intercalated by metal atoms, thereby tailoring the properties of bilayer borophene. Herein, we propose that sandwiched B/TM/B (TM=Co, Ni, Cu, Pd) could be a new 2D formation by transiton metal atoms intercalated into bilayer borophene network, it is quiet robust with both energetic, structural and thermal stability, and exhibits heat resistance of at least 1300 K. Besides, it is novel platform for electrocatalytic hydrogen evolution reaction (HER). The interecalation metal atom serves as single-atomic catalyst, which acting the nonmetal boron layers. Beyond that, the transtion metal is protected by outside boron layers from being corroded by acidic/alkaline solution. B/Cux/B, B/Pdx/B and B/Alx/B with different metal coverage exhibit defect-independent extremely low HER free energy in the range of -0.162 ~ 0.179 eV, -0.134 ~ 0.183 eV and -0.082 ~ 0.086 eV which are comparable to noble metal Pt. Combining excellent conduction, high structural and thermal stability, low resistance to intercalated behaviour, effortless water splitting process, excellent defect-independent catalytic performance, cheapness and abundance of raw materials, free of corrodation, 2D sandwiched B/TM/B (TM=Co, Ni, Cu, Pd) is believed to promising for electrocatalytic HER applications.",2309.02963v1 2023-11-22,Rashba-splitting-induced topological flat band detected by anomalous resistance oscillations beyond the quantum limit in ZrTe$_5$,"Topological flat band, on which the kinetic energy of topological electrons is quenched, represents a platform for investigating the topological properties of correlated systems. Recent experimental studies on flattened electronic bands have mainly concentrated on 2-dimensional materials created by van der Waals heterostructure-based engineering. Here, we report the observation of a topological flat band formed by polar-distortion-assisted Rashba splitting in a 3-dimensional Dirac material ZrTe$_5$. The polar distortion and resulting Rashba splitting on the band are directly detected by torque magnetometry and the anomalous Hall effect, respectively. The local symmetry breaking further flattens the band, on which we observe resistance oscillations beyond the quantum limit. These oscillations follow the temperature dependence of the Lifshitz-Kosevich formula but are evenly distributed in B instead of 1/B in high magnetic fields. Furthermore, the cyclotron mass anomalously gets enhanced about 10$^2$ times at field ~20 T. These anomalous properties of oscillations originate from a topological flat band with quenched kinetic energy. The topological flat band, realized by polar-distortion-assisted Rashba splitting in the 3-dimensional Dirac system ZrTe$_5$, signifies an intrinsic platform without invoking moir\'e or order-stacking engineering, and also opens the door for studying topologically correlated phenomena beyond the dimensionality of two.",2311.13346v2 2024-04-19,Machine Learning-guided accelerated discovery of structure-property correlations in lean magnesium alloys for biomedical applications,"Magnesium alloys are emerging as promising alternatives to traditional orthopedic implant materials thanks to their biodegradability, biocompatibility, and impressive mechanical characteristics. However, their rapid in-vivo degradation presents challenges, notably in upholding mechanical integrity over time. This study investigates the impact of high-temperature thermal processing on the mechanical and degradation attributes of a lean Mg-Zn-Ca-Mn alloy, ZX10. Utilizing rapid, cost-efficient characterization methods like X-ray diffraction and optical, we swiftly examine microstructural changes post-thermal treatment. Employing Pearson correlation coefficient analysis, we unveil the relationship between microstructural properties and critical targets (properties): hardness and corrosion resistance. Additionally, leveraging the least absolute shrinkage and selection operator (LASSO), we pinpoint the dominant microstructural factors among closely correlated variables. Our findings underscore the significant role of grain size refinement in strengthening and the predominance of the ternary Ca2Mg6Zn3 phase in corrosion behavior. This suggests that achieving an optimal blend of strength and corrosion resistance is attainable through fine grains and reduced concentration of ternary phases. This thorough investigation furnishes valuable insights into the intricate interplay of processing, structure, and properties in magnesium alloys, thereby advancing the development of superior biodegradable implant materials.",2404.13022v1 2010-02-08,Processing and Characterization of Multiferroic Bi-relaxors,"We compare chemical solution deposition (CSD), and pulsed-laser-deposition (PLD), specimens of the new room-temperature, single-phase, multiferroic magnetoelectric, [PbFe2/3W1/3O3]x[PbZr0.53Ti0.47O3]1-x (PZTFWx ~ 0.40 375{\deg}C , and a trade-off between reduced impurity concentration and structural degradation caused by plasma bombardment is achieved for 25s plasma exposure. 85 nm thick TiN films grown at a substrate temperature of 450{\deg}C, compatible with CMOS processes, with 0.5s chemisorption time and 25s plasma exposure exhibited a high plasmonic figure of merit (|{\epsilon}^'/{\epsilon}^''|) of 2.8 and resistivity of 31 {\mu}{\Omega}-cm. These TiN thin films fabricated with subwavelength apertures were shown to exhibit extraordinary transmission.",2001.05063v1 2021-06-26,High Infrared Reflectance Modulation in VO2 Films Synthesized on Glass and ITO coated Glass substrates using Atmospheric Oxidation of Vanadium,"Vanadium Dioxide (VO2) is a strongly correlated material, which exhibits insulator to metal transition at ~68 C along with large resistivity and infrared optical reflectance modulation. In this work, we use atmospheric pressure thermal oxidation of Vanadium to synthesize VO2 films on glass and ITO coated glass substrates. With the optimized short oxidation durations of 2 min and 4 min, the synthesized VO2 film shows high optical reflectance switching in long-wavelength infrared on glass substrates and mid-wavelength infrared on ITO coated glass substrates, respectively. Peak reflectance switching values of ~76% and ~79% are obtained on the respective substrates, which are among the highest reported values. Using the reflectance data, we extract VO2 complex refractive index in infrared wavelengths, in both the insulating and metallic phases. The extracted refractive index shows good agreement with VO2 synthesized using other methods. This demonstration of high optical reflectance switching in VO2 thin films, grown on low cost glass and ITO coated glass substrates, using a simple low thermal budget process will aid in enhancing VO2 applications in the optical domain.",2106.14006v1 2022-04-11,Emergent superconductivity in van der Waals Kagome material Pd3P2S8 under high pressure,"Kagome lattice systems have been proposed to host rich physics, which provide an excellent platform to explore unusual quantum states. Here, we report on the discovery of superconductivity in van der Waals material Pd3P2S8 under pressure. The superconductivity is observed in Pd3P2S8 for those pressures where the temperature dependence of the resistivity changes from a semiconducting-like behavior to that of a normal metal. The superconducting transition temperature Tc increases with applied pressure and reaches ~ 6.83 K at 79.5 GPa. Combining high-pressure XRD, Raman spectroscopy and theoretical calculations, our results demonstrate that the observed superconductivity induced by high pressure in Pd3P2S8 is closely related to the formation of amorphous phase, which results from the structural instability due to the enhanced coupling between interlayer Pd and S atoms upon compression.",2204.05179v1 2001-07-21,Distinct origins of magnetic -field -induced resistivity irreversibility in two manganites with similar ground states : Pr$_{0.5}$Sr$_{0.41}$Ca$_{0.09}$MnO$_{3}$ and La$_{0.5}$Ca$_{0.5}$MnO$_{3}$,"Our investigation of the magnetotransport in two charge ordered manganites with similar magnetic ground states reveals that the origin of magnetoresistance can not be concluded from the isofield resistivity, $\rho $(T, constant H), measurements alone. Both Pr$_{0.5}$Sr$_{0.41}$Ca$_{0.09}$MnO$_{3}$ (PrSrCa) and La$_{0.5}$Ca$_{0.5}$MnO$_{3}$ (LaCa) show a ferromagnetic transition (T$_{C}$ = 260 K for PrSrCa, 230 K for LaCa) followed by an antiferromagnetic transition (T$_{N}$ = 170 K for PrSrCa, 140 K for LaCa). These compounds show qualitatively similar magnetotransport : Below the irreversibility temperature T$_{IR}$, field cooled (FC) resistivity is lower than zero field cooled (ZFC) and decreases continuously with T, whereas the ZFC $\rho $(T, H) resembles $\ $the behavior of $\rho $(T, H = 0 T). The value of $\rho $(ZFC)/$\rho $(FC) is $\approx $ 10$^{4}$ at 5 K and $\mu_{0}$H = 7 T in both compounds. However, isothermal magnetic measurements suggest distinct origins of magnetoresistance : Field cooling enhances ferromagnetic phase fraction in LaCa whereas it drives PrSrCa into a metastable state with high magnetization. The distinct origins of magnetotransport is also reflected in other magnetic history dependent properties.",0107448v1 2006-09-15,Magneto Transport of high TCR (temperature coefficient of resistance) La2/3Ca1/3MnO3: Ag Polycrystalline Composites,"We report the synthesis, (micro)structural, magneto-transport and magnetization of polycrystalline La2/3Ca1/3MnO3:Agx composites with x = 0.0, 0.1, 0.2, 0.3 and 0.4. The temperature coefficient of resistance (TCR) near ferromagnetic (FM) transition is increased significantly with addition of Ag. The FM transition temperature (TFM) is also increased slightly with Ag addition. Magneto-transport measurements revealed that magneto-resistance MR is found to be maximum near TFM. Further the increased MR of up to 60% is seen above 300 K for higher silver added samples in an applied field of 7 Tesla. Sharp TCR is seen near TFM with highest value of up to 15 % for Ag (0.4) sample, which is an order of magnitude higher than as for present pristine sample and best value yet reported for any polycrystalline LCMO compound. Increased TCR, TFM and significant above room temperature MR of La2/3Ca1/3MnO3:Agx composites is explained on the basis of improved grains size and connectivity with silver addition in the matrix. Better coupled FM domains and nearly conducting grain boundaries give rise to improved physical properties of the La2/3Ca1/3MnO3 manganites.",0609364v1 2007-09-05,Microwave surface resistance of pristine and neutron-irradiated MgB2 samples in magnetic field,"We report on the microwave surface resistance of two polycrystalline Mg11B2 samples; one consists of pristine material, the other has been irradiated at very high neutron fluence. It has already been reported that in the strongly irradiated sample the two gaps merge into a single value. The mw surface resistance has been measured in the linear regime as a function of the temperature and the DC magnetic field, at increasing and decreasing fields. The results obtained in the strongly irradiated sample are quite well justified in the framework of a generalized Coffey and Clem model, in which we take into account the field distribution inside the sample due to the critical state. The results obtained in the pristine sample show several anomalies, especially at low temperatures, which cannot be justified in the framework of standard models for the fluxon dynamics. Only at temperatures near Tc and for magnetic fields greater than 0.5Hc2(T) the experimental data can quantitatively be accounted for by the Coffey and Clem model, provided that the upper-critical-field anisotropy is taken into due account.",0709.0618v2 2008-02-12,Two-Fluid Behaviour at the Origin of the Resistivity Peak in Doped Manganites,"We report a series of magnetic and transport measurements on high-quality single crystal samples of colossal magnetoresistive manganites, La_{0.7} Ca_{0.3} Mn O_3 and Pr_{0.7} Sr_{0.3} Mn O_3. 1 % Fe doping allows a Moessbauer spectroscopy study, which shows (i) unusual line broadening within the ferromagnetic phase and (ii) a coexistence of ferro- and paramagnetic contributions in a region, T_1T_2. This shows that phase separation into metallic (ferromagnetic) and insulating (paramagnetic) phases cannot be generally responsible for the resistivity peak (and hence for the associated colossal magnetoresistance). Our results can be understood phenomenologically within the two-fluid approach, which also allows for a difference between T_C and T_{MI}. Our data indeed imply that while magnetic and transport properties of the manganites are closely interrelated, the two transitions at T_C and T_{MI} can be viewed as distinct phenomena.",0802.1664v3 2008-06-15,Anisotropy in the electrical resistivity and susceptibility of superconducting BaFe$_{2}$As$_{2}$ single crystals,"Sizable single crystals of $BaFe_2As_2$ have been grown with self-flux method. The crystals are plate-like with c-axis perpendicular to the plane. The size can be as large as 3 x 5 x 0.2 $mm^3$. The resistivity anisotropy ($\rho_c/\rho_{ab}$) is as large as about 150, and independent of temperature. The transport in ab plane and along c-axis direction shares the same scattering mechanism. In contrast to the magnetic behavior of polycrystalline samples, no Curie-Weiss behavior are observed, a temperature linear dependent susceptibility occurs above spin-density-wave (SDW) transition. The susceptibility behavior is very similar to that of antiferromagnetic SDW chromium. Magnetic behavior of single crystal definitely gives evidence for existence of local moment except for the contribution to susceptibility from itinerant electrons. A resistivity minimum strongly dependent on magnetic field is observed. A log(1/T) divergency, similar to that of the underdoped cuprates, happens at low temperature. Here we first present intrinsic transport and magnetic properties, and their anisotropy from high quality single crystal.",0806.2452v2 2008-10-01,Qualitative explanation of the temperature behaviors of the transport properties and magnetic susceptibility of high-temperature superconductors in the normal state,"A model based on the alternating structure of the imbedded conduction layers (the Cu-O2 planes) with the charge-transfer-insulator (CTI) layers is proposed. There are three kinds of carriers, each with a different behavior: conduction-like holes in the Cu-O2 layers and electrons and normal holes in the CTI matrix between the Cu-O2 layers. This structure explains the strong anisotropies. The relationship is obtained between the concentration nq of conduction-like holes in the Cu-O2 layers and the temperature T. The anomalous temperature behavior of the resistivity as well as the Hall constant also follows. We give the hole density in ab plane a definite physical meaning, and also define explicitly optimal doping, overdoping and underdoping. Our model gives the correct temperature dependence of the resistivity and the hole constant on optimal doping, overdoping and underdoping, and it predicts the temperature behavior of the cotangent of the Hall angle quite well. Based on this model, we can also understand that the HiTc materials become ""Fermi Liquids"" in the extremely overdoped region, and the dR/dT becomes negative below some temperature T<1.211T0 in the underdoped case. Based on this model, the thermal behaviors of the magnetic susceptibility in different doping can also be easily explained. The resistivity along c-axis is discussed.",0810.0169v2 2011-01-29,"Crystal structure, physical properties and superconductivity in $A_{x}$Fe$_2$Se$_2$ single crystals","We studied the correlation among structure and transport properties and superconductivity in the different $A_x$Fe$_2$Se$_2$ single crystals ($A$ = K, Rb, and Cs). Two sets of (00$l$) reflections are observed in the X-ray single crystal diffraction patterns, and arise from the intrinsic inhomogeneous distribution of the intercalated alkali atoms. The occurrence of superconductivity is closely related to the {\sl c}-axis lattice constant, and the $A$ content is crucial to superconductivity. The hump observed in resistivity seems to be irrelevant to superconductivity. There exist many deficiencies within the FeSe layers in $A_x$Fe$_2$Se$_2$, while their $T_{\rm c}$ does not change so much. In this sense, superconductivity is robust to the Fe and Se vacancies. Very high resistivity in the normal state should arise from such defects in the conducting FeSe layers. $A_x$Fe$_2$Se$_2$ ($A$ = K, Rb, and Cs) single crystals show the same susceptibility behavior in the normal state, and no anomaly is observed in susceptibility at the hump temperature in resistivity. The clear jump in specific heat for Rb$_x$Fe$_2$Se$_2$ and K$_x$Fe$_2$Se$_2$ single crystals shows the good bulk superconductivity in these crystals.",1101.5670v1 2011-03-04,Measurements of thermodynamic and transport properties of EuC$_2$: a low-temperature analogue of EuO,"EuC$_2$ is a ferromagnet with a Curie-temperature of $T_C \simeq 15\,$K. It is semiconducting with the particularity that the resistivity drops by about 5 orders of magnitude on cooling through $T_C$, which is therefore called a metal-insulator transition. In this paper we study the magnetization, specific heat, thermal expansion, and the resistivity around this ferromagnetic transition on high-quality EuC$_2$ samples. At $T_C$ we observe well defined anomalies in the specific heat $c_p(T)$ and thermal expansion $\alpha(T)$ data. The magnetic contributions of $c_p(T)$ and $\alpha(T)$ can satisfactorily be described within a mean-field theory, taking into account the magnetization data. In zero magnetic field the magnetic contributions of the specific heat and thermal expansion fulfill a Gr\""uneisen-scaling, which is not preserved in finite fields. From an estimation of the pressure dependence of $T_C$ via Ehrenfest's relation, we expect a considerable increase of $T_C$ under applied pressure due to a strong spin-lattice coupling. Furthermore the influence of weak off stoichiometries $\delta$ in EuC$_{2 \pm \delta}$ was studied. It is found that $\delta$ strongly affects the resistivity, but hardly changes the transition temperature. In all these aspects, the behavior of EuC$_2$ strongly resembles that of EuO.",1103.0980v1 2012-07-13,Synthesis and acid resistance of maya blue pigment,"Maya blue is an organo-clay artificial pigment composed of indigo and palygorskite. It was invented and frequently used in Mesoamerica in ancient times (eighth to 16th centuries). We analyse in this paper one of the characteristics of Maya blue that has attracted the attention of scientists since its rediscovery in 1931: its high stability against chemical aggression (acids, alkalis, solvents, etc.) and biodegradation, which has permitted the survival of many works of art for centuries in hostile environments, such as the tropical forest. We have reproduced the different methods proposed to produce a synthetic pigment with the characteristics of the ancient Maya blue. The stability of the pigments produced using either palygorskite or sepiolite has been analysed by performing acid attacks of different intensities. The results are analysed in terms of pigment decolouration and destruction of the clay lattice, revealed by X-ray diffraction. Palygorskite pigments are much more resistant than sepiolite pigments. It is shown that indigo does not protect the clay lattice against acid aggression. We show that Maya blue is an extremely resistant pigment, but it can be destroyed using very intense acid treatment under reflux.",1207.3229v1 2013-04-07,Quasi-classical physics and T-linear resistivity in both strongly correlated and ordinary metals,"We show that near a quantum critical point generating quantum criticality of strongly correlated metals where the density of electron states diverges, the quasi-classical physics remains applicable to the description of the resistivity \rho of strongly correlated metals due to the presence of a transverse zero-sound collective mode, reminiscent of the phonon mode in solids. We demonstrate that at T, being in excess of an extremely low Debye temperature T_D, the resistivity \rho(T) changes linearly with T, since the mechanism, forming the T dependence of \rho(T), is the same as the electron-phonon mechanism that prevails at high temperatures in ordinary metals. Thus, electron-phonon scattering leads to near material-independence of the lifetime \tau of quasiparticles that is expressed as the ratio of the Planck constant \hbar to the Boltzmann constant k_B, T\tau\sim \hbar/k_B. We find that at T 10^{4}}$), high detection efficiency, and position resolution exceeding 100 $\mu$m. The spark current was suppressed, and the new resistive $\mu$-PIC was operated stably under fast-neutrons irradiation. These features offer solutions for a charged-particle-tracking detector in future high-rate applications.",1901.03836v1 2015-10-13,Interface-mediated thermomechanical effects during high velocity impact between monocrystalline surfaces,"High velocity impact between crystalline surfaces is important for a range of material phenomena, yet a fundamental understanding of the effect of surface structure, energetics and kinetics on the underlying thermo-mechanical response remains elusive. Here, we employ non-equilibrium molecular dynamics (NEMD) simulations to describe the nanoscale dynamics of the high velocity impact between commensurate and incommensurate monocrystalline (001) copper surfaces. For impact velocities in the range 100-1200 m/s, the kinetic energy dissipation involves nucleation and emission of dislocation loops from defective sites within the rapidly forming interface, well below the bulk single-crystal yield point. At higher velocities, adiabatic dissipation occurs via plasticity-induced heating as the interface structurally melts following the impact. The adhesive strength of the reformed interface is controlled by the formation and nucleation of dislocations and point defects as they modify the interfacial energy relative to the deformed bulk. As confirmation, the excess interface energy decreases monotonically with increasing impact velocity. The relative crystal orientation of the surfaces equally important; the grain boundaries formed following incommensurate impact exhibit higher impact resistance, with smaller defect densities and interfacial enthalpies, suggesting an enhanced ability of the grain boundaries to absorb the non-equilibrium damage and therefore facilitate particle bonding. Our study highlights the key role played by the atomic-scale surface structure in determining the impact resistance and adhesion of crystalline surfaces.",1510.03775v1 2007-10-03,Directional-dependent thermally activated motion of vortex bundles and theory of anomalous Hall effect in type-II conventional and high-Tc superconductors,"The anomalous Hall effect for type-II conventional and high-Tc superconductors is studied based upon the theory of thermally activated motion of vortex bundles jumping over the directional-dependent energy barrier. It is shown that the Hall anomaly is universal for type-II conventional and high-Tc superconductors as well as for superconducting bulk materials and thin films, provided certain conditions are satisfied. We find that the directional-dependent potential barrier of the vortex bundles renormalizes the Hall and longitudinal resistivities, and Hall anomaly for superconductors is induced by the competition between the Magnus force and the random collective pinning force of the vortex bundle. We also find that the domain of anomalous Hall effect includes two regions: the region of thermally activated motion of the small vortex bundles and that of the large vortex bundles separated by the contour of the quasiorder-disorder first-order phase transition, or the peak effect of the vortex system. The Hall and longitudinal resistivities as functions of temperature as well as applied magnetic field have been calculated for type-II superconducting films and bulk materials. The conditions for occurring the double sign reversal or reentry phenomenon is also investigated. All the results are in agreement with the experiments.",0710.0700v2 2022-04-20,Superconducting bimodal ionic photo-memristor,"Memristive circuit elements constitute a cornerstone for novel electronic applications, such as neuromorphic computing, called to revolutionize information technologies. By definition, memristors are sensitive to the history of electrical stimuli, to which they respond by varying their electrical resistance across a continuum of nonvolatile states. Recently, much effort has been devoted to developing devices that present an analogous response to optical excitation. Here we realize a new class of device, a tunnelling photo-memristor, whose behaviour is bimodal: both electrical and optical stimuli can trigger the switching across resistance states in a way determined by the dual optical-electrical history. This unique behaviour is obtained in a device of ultimate simplicity: an interface between a high-temperature superconductor and a transparent semiconductor. The microscopic mechanism at play is a reversible nanoscale redox reaction between both materials, whose oxygen content determines the electron tunnelling rate across their interface. Oxygen exchange is controlled here via illumination by exploiting a competition between electrochemistry, photovoltaic effects and photo-assisted ion migration. In addition to their fundamental interest, the unveiled electro-optic memory effects have considerable technological potential. Especially in combination with high-temperature superconductivity which, beyond facilitating the high connectivity required in neuromorphic circuits, brings photo-memristive effects to the realm of superconducting electronics.",2204.09255v1 2018-11-03,Modern Data Analytics Approach to Predict Creep of High-Temperature Alloys,"A breakthrough in alloy design often requires comprehensive understanding in complex multi-component/multi-phase systems to generate novel material hypotheses. We introduce a modern data analytics workflow that leverages high-quality experimental data augmented with advanced features obtained from high-fidelity models. Herein, we use an example of a consistently-measured creep dataset of developmental high-temperature alloy combined with scientific alloy features populated from a high-throughput computational thermodynamic approach. Extensive correlation analyses provide ranking insights for most impactful alloy features for creep resistance, evaluated from a large set of candidate features suggested by domain experts. We also show that we can accurately train machine learning models by integrating high-ranking features obtained from correlation analyses. The demonstrated approach can be extended beyond incorporating thermodynamic features, with input from domain experts used to compile lists of features from other alloy physics, such as diffusion kinetics and microstructure evolution.",1811.01239v1 2021-01-24,Electronic structure and transport properties of sol-gel-derived high-entropy Ba(Zr0.2Sn0.2Ti0.2Hf0.2Nb0.2)O3 thin films,"High-entropy perovskite thin films, as the prototypical representative of the high-entropy oxides with novel electrical and magnetic features, have recently attracted great attention. Here, we reported the electronic structure and charge transport properties of sol-gel-derived high-entropy Ba(Zr0.2Sn0.2Ti0.2Hf0.2Nb0.2)O3 thin films annealed at various temperatures. By means of X-ray photoelectron spectroscopy and absorption spectrum, it is found that the conduction-band-minimum shifts downward and the valence-band-maximum shifts upward with the increase of annealing temperature, leading to the narrowed band gap. Electrical resistance measurements confirmed a semiconductor-like behavior for all the thin films. Two charge transport mechanisms, i.e., the thermally-activated transport mechanism at high temperatures and the activation-less transport mechanism at low temperatures, are identified by a self-consistent analysis method. These findings provide a critical insight into the electronic band structure and charge transport behavior of Ba(Zr0.2Sn0.2Ti0.2Hf0.2Nb0.2)O3, validating it as a compelling high-entropy oxide material for future electronic/energy-related technologies.",2101.09633v2 2015-06-16,Unforeseen high temperature and humidity stability of FeCl$_3$ intercalated few layer graphene,"We present the first systematic study of the stability of the structure and electrical properties of FeCl$_3$ intercalated few-layer graphene to high levels of humidity and high temperature. Complementary experimental techniques such as electrical transport, high resolution transmission electron microscopy and Raman spectroscopy conclusively demonstrate the unforeseen stability of this transparent conductor to a relative humidity up to $100 \%$ at room temperature for 25 days, to a temperature up to $150\,^\circ$C in atmosphere and up to a temperature as high as $620\,^\circ$C in vacuum, that is more than twice higher than the temperature at which the intercalation is conducted. The stability of FeCl$_3$ intercalated few-layer graphene together with its unique values of low square resistance and high optical transparency, makes this material an attractive transparent conductor in future flexible electronic applications.",1506.04907v1 2009-12-24,Properties of MgB2 bulk,"The review considers bulk MgB2-based materials in terms of their structure, superconducting and mechanical properties. Superconducting transition temperatures of 34.5-39.4 K, critical current densities of 1.8-1.0 x E6 A/sq.cm in self field and 103 in 8 T field at 20 K, 3-1.5xE5 A/sq. cm in self field at 35 K, HC2 15 T at 22 K and Hirr 13 T at 20 K have been registered for polycrystalline materials. As TEM and SEM study show, dispersed higher borides and rather big amount (5-14 percents) of oxygen (bonded simultaneously with Mg and B) can be present in the structure even if X-ray pattern contains only reflexes of well crystallized MgB2 with traces of MgO. Materials with such a rather high oxygen content demonstrated high superconducting characteristics. At present it is established that nanosized MgB12 grains provide effective pinning in polycrystalline material. Besides, additions can introduce the MgB2 structure inducing disorder in lattice sites (for example, C substitution for B). The disorder increases the normal state resistivity, magnetic penetration depth, and the upper critical field, but reduces the transition temperature and anisotropy. It is highly probable that the additives (Ti, Ta, Zr, SiC) together with synthesis or sintering temperature can affect the distribution of oxygen and hydrogen in the material structure as well as the formation of grains of higher borides, thus influencing superconducting properties. The superconductivity of materials with matrix close to MgB12 in stoichiometry (Tc=37 K) has been defined.",0912.4906v1 2017-10-23,Realization of a hole-doped Mott insulator on a triangular silicon lattice,"The physics of doped Mott insulators is at the heart of some of the most exotic physical phenomena in materials research including insulator-metal transitions, colossal magneto-resistance, and high-temperature superconductivity in layered perovskite compounds. Advances in this field would greatly benefit from the availability of new material systems with similar richness of physical phenomena, but with fewer chemical and structural complications in comparison to oxides. Using scanning tunneling microscopy and spectroscopy, we show that such a system can be realized on a silicon platform. Adsorption of one-third monolayer of Sn atoms on a Si(111) surface produces a triangular surface lattice with half-filled dangling bond orbitals. Modulation hole-doping of these dangling bonds unveils clear hallmarks of Mott physics, such as spectral weight transfer and the formation of quasi-particle states at the Fermi level, well-defined Fermi contour segments, and a sharp singularity in the density of states. These observations are remarkably similar to those made in complex oxide materials, including high-temperature superconductors, but highly extraordinary within the realm of conventional sp-bonded semiconductor materials. It suggests that exotic quantum matter phases can be realized and engineered on silicon-based materials platforms.",1710.08065v1 2020-04-12,Investigation on the Mechanical Properties of Functionally Graded Nickel and Aluminium Alloy by Molecular Dynamics Study,"Functionally graded materials (FGMs), have drawn considerable attention of the worldwide researchers and scientific community because of its unique mechanical, thermal and electrical properties which may be exploited by varying the compositions gradually over volume. This makes FGM multifunctional material (properties changing continuously in a certain direction) for specific purpose without creating any phase interface thus making it superior to its composite counterparts. In this paper, we applied Molecular Dynamics (MD) approach to investigate the mechanical properties of functional graded Ni-Al alloy with Ni coating by applying uniaxial tension. Nickel-Aluminum (Ni-Al) alloy has been used extensively in the industry due to its remarkable mechanical and thermal properties. Our aim is to find the difference in material behavior when we change the grading function (linear, elliptical and parabolic), temperature and crystallographic direction. We also observe distinct type of failure mechanism for different grading function at different temperature. Close observation reveals that elliptically graded Ni-Al alloy has high tensile strength at low temperature whereas at high temperature, the highest tensile strength is found for parabolic grading. Besides, at any temperature, the parabolically graded Ni-Al alloy shows superior elasticity than its elliptical and linear counterpart. Moreover, it is also observed that [111] crystallographic direction for this alloy demonstrates more resistivity towards failure than any other crystallographic direction. It is found that lattice disorder plays a significant role on the mechanical properties of Functionally Graded Materials (FGMs). This paper details a pathway to tune the mechanical properties like Young's Modulus, plasticity and yield strength at molecular level by varying the composition of materials along different grading functions.",2004.05651v1 1997-03-03,Longitudinal and transverse dissipation in a simple model for the vortex lattice with screening,"Transport properties of the vortex lattice in high temperature superconductors are studied using numerical simulations in the case in which the non-local interactions between vortex lines are dismissed. The results obtained for the longitudinal and transverse resistivities in the presence of quenched disorder are compared with the results of experimental measurements and other numerical simulations where the full interaction is considered. This work shows that the dependence on temperature of the resistivities is well described by the model without interactions, thus indicating that many of the transport characteristics of the vortex structure in real materials are mainly a consequence of the topological configuration of the vortex structure only. In addition, for highly anisotropic samples, a regime is obtained where longitudinal coherence is lost at temperatures where transverse coherence is still finite. I discuss the possibility of observing this regime in real samples.",9703035v1 1997-08-19,Metallization of Fluid Hydrogen,"The electrical resistivity of liquid hydrogen has been measured at the high dynamic pressures, densities and temperatures that can be achieved with a reverberating shock wave. The resulting data are most naturally interpreted in terms of a continuous transition from a semiconducting to a metallic, largely diatomic fluid, the latter at 140 GPa, (ninefold compression) and 3000 K. While the fluid at these conditions resembles common liquid metals by the scale of its resistivity of 500 micro-ohm-cm, it differs by retaining a strong pairing character, and the precise mechanism by which a metallic state might be attained is still a matter of debate. Some evident possibilities include (i) physics of a largely one-body character, such as a band-overlap transition, (ii) physics of a strong-coupling or many-body character,such as a Mott-Hubbard transition, and (iii) processes in which structural changes are paramount.",9708144v1 1997-09-16,The Metallic-Like Conductivity of a Two-Dimensional Hole System,"We report on a zero magnetic field transport study of a two-dimensional, variable-density, hole system in GaAs. As the density is varied we observe, for the first time in GaAs-based materials, a crossover from an insulating behavior at low-density, to a metallic-like behavior at high-density, where the metallic behavior is characterized by a large drop in the resistivity as the temperature is lowered. These results are in agreement with recent experiments on Si-based two-dimensional systems by Kravchenko et al. and others. We show that, in the metallic region, the resistivity is dominated by an exponential temperature-dependence with a characteristic temperature which is proportional to the hole density, and appear to reach a constant value at lower temperatures.",9709184v3 1998-04-23,Hysteretic behavior and evidence for domain formation in a double-layer quantum Hall system at total filling factor 2,"We report anomalous behavior in a double-layer two dimensional hole gas (2DHG) at even integer filling factors which includes hysteresis in the longitudinal and Hall resistances and a very weak temperature dependence of the resistance minima. All anomalies disappear and the conventional quantum Hall effect behavior recovers when a thin metal film is placed on top of the 2DHG. The behavior is attributed to presence of the theoretically predicted magnetic ordering at even integer filling factors which causes the formation of macroscopic spin-charge domains.",9804256v2 1998-11-18,Hall-effect in LuNi_2B_2C in normal and superconducting mixed states,"The Hall resistivity rho_{xy} of LuNi_2B_2C is negative in the normal as well as in the mixed state and has no sign reversal typical for high-T_c superconductors. A distinct nonlinearity in the rho_{xy} dependence on field H was found in the normal state for T < 40K, accompanied by a large magnetoresistance reaching +90% for mu_0H=16T at T=20K. The scaling relation rho_{xy} ~ \rho_{xx}^\beta (\rho_{xx} is the longitudinal resistivity) was found in the mixed state, the value of \beta being dependent on the degree of disorder.",9811273v1 1999-07-22,Charge carrier density collapse in La_0.67Ca_0.33MnO_3 and La_0.67Sr_0.33MnO_3 epitaxial thin films,"We measured the temperature dependence of the linear high field Hall resistivity of La_0.67Ca_0.33MnO_3 (T_C=232K) and La_0.67Sr_0.33MnO_3 (T_C=345K) thin films in the temperature range from 4K up to 360K in magnetic fields up to 20T. At low temperatures we find a charge carrier density of 1.3 and 1.4 holes per unit cell for the Ca- and Sr-doped compound, respectively. In this temperature range electron-magnon scattering contributes to the longitudinal resistivity. At the ferromagnetic transition temperature T_C a dramatic drop in the number of current carriers $n$ down to 0.6 holes per unit cell, accompanied by an increase in unit cell volume, is observed. Corrections of the Hall data due to a non saturated magnetic state will lead a more pronounced charge carrier density collapse.",9907346v1 1999-08-05,Fermi-level alignment at metal-carbon nanotube interfaces: application to scanning tunneling spectroscopy,"At any metal-carbon nanotube interface there is charge transfer and the induced interfacial field determines the position of the carbon nanotube band structure relative to the metal Fermi-level. In the case of a single-wall carbon nanotube (SWNT) supported on a gold substrate, we show that the charge transfers induce a local electrostatic potential perturbation which gives rise to the observed Fermi-level shift in scanning tunneling spectroscopy (STS) measurements. We also discuss the relevance of this study to recent experiments on carbon nanotube transistors and argue that the Fermi-level alignment will be different for carbon nanotube transistors with low resistance and high resistance contacts.",9908073v3 1999-08-25,Hall effect of epitaxial double-perovskite Sr_2FeMoO_6 thin films,"We prepared high epitaxial thin films of the compound Sr_2FeMoO_6 with narrow rocking curves by pulsed laser deposition. The diagonal and nondiagonal elements of the resistivity tensor were investigated at temperatures from 4 K up to room temperature in magnetic fields up to 8 T. An electronlike ordinary Hall effect and a holelike anomalous Hall contribution are observed. Both coefficients have reversed sign compared to the colossal magnetoresistive manganites. We found at 300 K an ordinary Hall coefficent of -1.87x10^{-10} m^3/As, corresponding to a nominal charge carrier density of four electrons per formula unit. At low temperature only a small negative magnetoresistance is observed which vanishes at higher temperatures. The temperature coefficient of the resistivity is negative over the whole temperature range. A Kondo like behavior is observed below 30 K while above 100 K variable range hopping like transport occurs.",9908361v2 1999-10-15,Electronic Transport in a Three-dimensional Network of 1-D Bismuth Quantum Wires,"The resistance R of a high density network of 6 nm diameter Bi wires in porous Vycor glass is studied in order to observe its expected semiconductor behavior. R increases from 300 K down to 0.3 K. Below 4 K, where R varies approximately as ln(1/T), the order-of-magnitude of the resistance rise, as well as the behavior of the magnetoresistance are consistent with localization and electron-electron interaction theories of a one-dimensional disordered conductor in the presence of strong spin-orbit scattering. We show that this behaviour and the surface-enhanced carrier density may mask the proposed semimetal-to-semiconductor transition for quantum Bi wires.",9910241v1 2000-01-25,Pressure Induced Quantum Critical Point and Non-Fermi-Liquid Behavior in BaVS3,"The phase diagram of BaVS3 is studied under pressure using resistivity measurements. The temperature of the metal to nonmagnetic Mott insulator transition decreases under pressure, and vanishes at the quantum critical point p_cr=20kbar. We find two kinds of anomalous conducting states. The high-pressure metallic phase is a non-Fermi liquid described by Delta rho = T^n where n=1.2-1.3 at 1K < T < 60K. At p0.125. Resistivity measurements in magnetic fields parallel and perpendicular to the basal plane of the crystals showed a nearly isotropic state in the heavily-doped crystals (x>0.1).",0305485v1 2003-07-01,Efficient nonlinear room-temperature spin injection from ferromagnets into semiconductors through a modified Schottky barrier,"We suggest a consistent microscopic theory of spin injection from a ferromagnet (FM) into a semiconductor (S). It describes tunneling and emission of electrons through modified FM-S Schottky barrier with an ultrathin heavily doped interfacial S layer . We calculate nonlinear spin-selective properties of such a reverse-biased FM-S junction, its nonlinear I-V characteristic, current saturation, and spin accumulation in S. We show that the spin polarization of current, spin density, and penetration length increase with the total current until saturation. We find conditions for most efficient spin injection, which are opposite to the results of previous works, since the present theory suggests using a lightly doped resistive semiconductor. It is shown that the maximal spin polarizations of current and electrons (spin accumulation) can approach 100% at room temperatures and low current density in a nondegenerate high-resistance semiconductor.",0307030v4 2003-12-23,1-D Simulation of the Electron Density Distribution in a Novel Nonvolatile Resistive Random Access Memory Device,"The operation of a novel nonvolatile memory device based on a conductive ferroelectric/non-ferroelectric thin film multilayer stack is simulated numerically. The simulation involves the self-consistent steady state solution of Poisson's equation and the transport equation for electrons assuming a Drift-Diffusion transport mechanism. Special emphasis is put on the screening of the spontaneous polarization by conduction electrons as a function of the applied voltage. Depending on the orientation of the polarization in the ferroelectric layer, a high and a low resistive state are found giving rise to a hysteretic I-V characteristic. The R_high to R_low ratio ranging from > 50% to several orders of magnitude is calculated as a function of the dopant content.",0312609v1 2004-03-08,"Hole mobility in organic single crystals measured by a ""flip-crystal"" field-effect technique","We report on single crystal high mobility organic field-effect transistors (OFETs) prepared on prefabricated substrates using a ""flip-crystal"" approach. This method minimizes crystal handling and avoids direct processing of the crystal that may degrade the FET electrical characteristics. A chemical treatment process for the substrate ensures a reproducible device quality. With limited purification of the starting materials, hole mobilities of 10.7, 1.3, and 1.4 cm^2/Vs have been measured on rubrene, tetracene, and pentacene single crystals, respectively. Four-terminal measurements allow for the extraction of the ""intrinsic"" transistor channel resistance and the parasitic series contact resistances. The technique employed in this study shows potential as a general method for studying charge transport in field-accumulated carrier channels near the surface of organic single crystals.",0403210v1 2004-04-11,Synthesis of as-grown superconducting MgB_2 thin films by molecular beam epitaxy in UHV conditions,"As-grown superconducting MgB_2 thin films have been grown on SrTiO_3(001), MgO(001), and Al_2O_3(0001) substrates by a molecular beam epitaxy (MBE) method with novel co-evaporation conditions of low deposition rate in ultra-high vacuum. The structural and physical properties of the films were studied by RHEED, XRD, electrical resistivity measurements, and SQUID magnetometer. The RHEED patterns indicate three-dimensional growth for MgB_2. The highest T_c determined by resistivity measurement was about 36K in these samples. And a clear Meissner effect below T_c was observed using magnetic susceptibility measurement. We will discuss the influence of B buffer layer on the structural and physical properties.",0404252v1 2004-08-20,Anomalous Hall effect in insulating Ga1-xMnxAs,"We have investigated the effect of doping by Te on the anomalous Hall effect in Ga1-xMnxAs (x = 0.085). For this relatively high value of x the temperature dependence of resistivity shows an insulating behavior. It is well known that in Ga1-xMnxAs the Mn ions naturally act as acceptors. Additional doping by Te donors decreases the Curie temperature and increases the anomalous Hall resistivity. With increasing Te concentration the long-range ferromagnetic order in Ga1-xMnxAs eventually disappears, and paramagnetic-to-spin glass transition is observed instead. The critical concentration of holes required for establishing ferromagnetic order in Ga1-xMnxAs (x = 0.085) has been estimated by using the magnetic polaron percolation theory proposed by Kaminski and Das Sarma [Phys.Rev.Lett. 88, 247202 (2002)].",0408446v1 2005-01-14,Magnetization and magnetoresistance in insulating phases of SrFeO3-d,"We report the synthesis and properties of two new insulating phases of SrFeO3-d with introduction of oxygen deficiencies in metallic SrFeO3 ; one with 0.15 < d < 0.19 (sample A)and the other above d = 0.19 (sample B). Sample A shows large negative magnetoresistance around the charged ordering (CO) temperature with magnetic anomalies seen in the temperature dependent resistivity,magnetization and M-H hysteresis loops. Sample B shows a smooth insulating behavior with no thermal hysteresis in the resistivity and with a small positive magnetoresistance. cac and cdc show multiple features associated with a frustrated magnetic order (helical) due to competing ferro- and antiferromagnetic interactions. The competing effects of ferro- and antiferromagnetic phases extend up to T ~ 230 K revealing a new high temperature scale in this system. These observations are discussed in the context of magnetic interactions associated with the varying Fe4+/Fe3+ ratio.",0501352v1 2005-07-14,Field-Dependent Hall Effect in Single Crystal Heavy Fermion YbAgGe below 1K,"We report the results of a low temperature (T >= 50 mK) and high field (H <= 180 kOe) study of the Hall resistivity in single crystals of YbAgGe, a heavy fermion compound that demonstrates field-induced non-Fermi-liquid behavior near its field-induced quantum critical point. Distinct features in the anisotropic, field-dependent Hall resistivity sharpen on cooling down and at the base temperature are close to the respective critical fields for the field-induced quantum critical point. The field range of the non-Fermi-liquid region decreases on cooling but remains finite at the base temperature with no indication of its conversion to a point for T -> 0. At the base temperature, the functional form of the field-dependent Hall coefficient is field direction dependent and complex beyond existing simple models thus reflecting the multi-component Fermi surface of the material and its non-trivial modification at the quantum critical point.",0507338v1 2005-10-20,Stick slip motion in grain grain friction in a humid atmosphere,"We set up an original apparatus to measure the grain grain friction stress inside a granular medium composed of sodo-silicate-glass beads surrounded by a water vapor atmosphere.We analyze here the influence of the physico chemistry of water on our glass beads and its consequences on our shear experiment. We found two scales in the analysis of the shear stress signal. On the microscopic scale of one bead, the experimental results show a dependence on the size of beads, on the shear rate and on humidity for the resulting stick slip signal. On the macroscopic scale of the whole assembly of beads, the behavior of the total amplitude of the shear stress depends on the size of the beads and is humidity dependent only for relative humidity larger than 80%. For high degrees of humidity, on the microscopic scale, water lubricates the surface of the beads leading to a decrease in the microscopic resistance to shear while on the macroscopic scale the resistance to shear is increased: the assembly of very humid grains behaves as a non Newtonian fluid.",0510532v1 2006-06-23,Electronic transport in Si nanowires: Role of bulk and surface disorder,"We calculate the resistance and mean free path in long metallic and semiconducting silicon nanowires (SiNWs) using two different numerical approaches: A real space Kubo method and a recursive Green's function method. We compare the two approaches and find that they are complementary: depending on the situation a preferable method can be identified. Several numerical results are presented to illustrate the relative merits of the two methods. Our calculations of relaxed atomic structures and their conductance properties are based on density functional theory without introducing adjustable parameters. Two specific models of disorder are considered: Un-passivated, surface reconstructed SiNWs are perturbed by random on-site (Anderson) disorder whereas defects in hydrogen passivated wires are introduced by randomly removed H atoms. The un-passivated wires are very sensitive to disorder in the surface whereas bulk disorder has almost no influence. For the passivated wires, the scattering by the hydrogen vacancies is strongly energy dependent and for relatively long SiNWs (L>200 nm) the resistance changes from the Ohmic to the localization regime within a 0.1 eV shift of the Fermi energy. This high sensitivity might be used for sensor applications.",0606600v1 2006-07-18,Dielectric breakdown in underoxidized magnetic tunnel junctions: Dependence on oxidation time and area,"Magnetic tunnel junctions (MTJs) with partially oxidized 9 \AA AlO$_x$-barriers were recently shown to have the necessary characteristics to be used as magnetoresistive sensors in high-density storage devices. Here we study dielectric breakdown in such underoxidized magnetic tunnel junctions, focusing on its dependence on tunnel junction area and oxidation time. A clear relation between breakdown mechanism and junction area is observed for the MTJs with the highest studied oxidation time: samples with large areas fail usually due to extrinsic causes (characterized by a smooth resistance decrease at dielectric breakdown). Small area junctions fail mainly through an intrinsic mechanism (sharp resistance decrease at breakdown). However, this dependence changes for lower oxidation times, with extrinsic breakdown becoming dominant. In fact, in the extremely underoxidized magnetic tunnel junctions, failure is exclusively related with extrinsic causes, independently of MTJ-area. These results are related with the presence of defects in the barrier (weak spots that lead to intrinsic breakdown) and of metallic unoxidized Al nanoconstrictions (leading to extrinsic breakdown).",0607452v1 2007-01-20,Fabrication and Low Temperature Thermoelectric Properties of Na_xCoO_2 (x = 0.68 and 0.75) Epitaxial Films by the Reactive Solid-Phase Epitaxy,"We have fabricated Na_xCoO_2 thin films via lateral diffusion of sodium into Co_3O_4 (111) epitaxial films (reactive solid-phase epitaxy: Ref. 4). The environment of thermal diffusion is key to the control of the sodium content in thin films. From the results of x-ray diffraction and in-plane resistivity, the epitaxial growth and the sodium contents of these films were identified. The thermoelectric measurements show a large thermoelectric power similar to that observed in single crystals. The quasiparticle scattering rate is found to approach zero at low temperatures, consistent with the small residual resistivity, indicating high quality of the Na_xCoO_2 thin films.",0701492v1 2007-02-05,Existence of two electronic states in Sr4Ru3O10 at low temperatures,"We report measurements on in-plane resistivity, thermopower, and magnetization as a function of temperature and magnetic fields on single crystalline Sr4Ru3O10 grown by the floating zone method. As the temperature was lowered to below around 30 K, the in-plane and c-axis resistivities and the thermopower were found to exhibit a step feature accompanied by hysteresis behavior when the in-plane field was swept up and down from below 10 kOe to above 20 kOe. The sharp increase in the thermopower with increasing in-plane magnetic field at low temperatures has not been observed previously in layered transition metal oxides. Comparing with magnetization data, we propose that the step feature marks the transition between the two different electronic states in Sr4Ru3O10. We propose that the alignment of domains by the in-plane magnetic field is responsible to the emergence of the new electronic states in high applied in-plane magnetic field.",0702093v1 2007-05-02,Comment on ``Collapse of Coherent Quasiparticle States in $θ$-(BEDT-TTF)$_2$I$_3$ Observed by Optical Spectroscopy'',"Recently, Takenaka et al. reported that the resistivity rho(T) of theta-(BEDT-TTF)_2I_3 (theta-ET) exceeds the Ioffe-Regel resistivity by a factor of 50 at large temperatures T (``bad metal''). This was ascribed to strong correlation. We argue that the optical conductivity sigma(omega) implies that correlation is not very strong, and that correlation gives no general strong suppression of sigma(omega). The large rho(T) is primarily due to a downturn in sigma(omega) at small omega, earlier emphasized by Takenaka et al. as the explanation for bad metal behavior of high-T_c cuprates. We argue, however, that for cuprates strong correlation is the main effect. The data of Takenaka et al. puts theta-ET in a new class of bad metals.",0705.0230v1 2007-07-15,Physical properties of a new cuprate superconductor Pr_2Ba_4Cu_7O_{15-δ},"We present studies of the thermal, magnetic and electrical transport properties of reduced polycrystalline Pr_2Ba_4Cu_7O_{15-\delta} (Pr247) showing a superconducting transition at Tc = 10 - 16 K and compare them with those of as-sintered non-superconducting Pr247. The electrical resistivity in the normal state exhibited T2 dependence up to approximately 150 K. A clear specific heat anomaly was observed at Tc for Pr247 reduced in a vacuum for 24 hrs, proving the bulk nature of the superconducting state. By the reduction treatment, the magnetic ordering temperature TN of Pr moments decreased from 16 to 11 K, and the entropy associated with the ordering increased, while the effective paramagnetic moments obtained from the DC magnetic susceptibility varied from 2.72 to 3.13 mB. The sign of Hall coefficient changed from positive to negative with decreasing temperature in the normal state of a superconducting Pr247, while that of as-sintered one was positive down to 5 K. The electrical resistivity under high magnetic fields was found to exhibit T^a dependence (a = 0.08 - 0.4) at low temperatures. A possibility of superconductivity in the so-called CuO double chains is discussed.",0707.2180v1 2007-07-30,Intrinsic tunneling in phase separated manganites,"We present evidence of direct electron tunneling across intrinsic insulating regions in sub-micrometer wide bridges of the phase separated ferromagnet (La,Pr,Ca)MnO$_3$. Upon cooling below the Curie temperature, a predominantly ferromagnetic supercooled state persists where tunneling across the intrinsic tunnel barriers (ITBs) results in metastable, temperature-independent, high-resistance plateaus over a large range of temperatures. Upon application of a magnetic field, our data reveal that the ITBs are extinguished resulting in sharp, colossal, low-field resistance drops. Our results compare well to theoretical predictions of magnetic domain walls coinciding with the intrinsic insulating phase.",0707.4411v2 2008-01-09,Impact of in-plane currents on magnetoresistance properties of an exchange-biased spin-valve with insulating antiferromagnetic layer,"The impact of in-plane alternating currents on the exchange bias, resistance, and magnetoresistance of a CoFe/NiCoO/CoFe/Cu/CoFe spin-valve is studied. With increasing current, the resistance is increased while the maximum magnetoresistance ratio decreases. Noticeably, the reversal of the pinned layer is systematically suppressed in both field sweeping directions. Since the NiCoO oxide is a good insulator, it is expected that the ac current flows only in the CoFe/Cu/CoFe top layers, thus ruling out any presence of spin-transfer torque acting on the spins in the antiferromagnetic layer. Instead, our measurements show clear evidences for the influence of Joule heating caused by the current. Moreover, results from temperature-dependent measurements very much resemble those of the current dependence, indicating that the effect of Joule heating plays a major role in the current-in-plane spin-valve configurations. The results also suggest that spin-transfer torques between ferromagnetic layers might still exist and compete with the exchange bias at sufficiently high currents.",0801.1515v1 2008-04-09,"Curie point singularity in the temperature derivative of resistivity in (Ga,Mn)As","We observe a singularity in the temperature derivative $d\rho/dT$ of resistivity at the Curie point of high-quality (Ga,Mn)As ferromagnetic semiconductors with $T_c$'s ranging from approximately 80 to 185 K. The character of the anomaly is sharply distinct from the critical contribution to transport in conventional dense-moment magnetic semiconductors and is reminiscent of the $d\rho/dT$ singularity in transition metal ferromagnets. Within the critical region accessible in our experiments, the temperature dependence on the ferromagnetic side can be explained by dominant scattering from uncorrelated spin fluctuations. The singular behavior of $d\rho/dT$ on the paramagnetic side points to the important role of short-range correlated spin fluctuations.",0804.1578v2 2008-06-24,Low temperature thermal resistance for a new design of silver sinter heat exchanger,"We have developed a novel procedure for constructing high surface area silver sinter heat exchangers. Our recipe incorporates nylon fibers having a diameter of ~ 50 microns and thin wires of bulk silver in the heat exchanger. In order to increase the thermal conductance of liquid helium within the heat exchanger, prior to sintering, the nylon fibers are dissolved with an organic acid leaving a network of channels. In addition, the silver wires reinforce the structural integrity, and reduce the resistance, of the silver sinter. We have constructed a 3-He melting curve thermometer (MCT) with this type of heat exchanger and measured the thermal time response of the liquid 3-He inside the MCT in the temperature range T = 2-150 mK. We find a thermal relaxation time of ~ 490 s at T ~ 1 mK. We have used scanning electron microscopy (SEM) to characterize the heat exchanger and BET absorption for determination of the specific surface area.",0806.3930v1 2008-08-09,Transport and Magnetic properties of Fe1/3VSe2,"Electrical conductivity, thermopower and magnetic properties of Fe-intercalated Fe0.33VSe2 has been reported between 4.2K - 300K. We observe a first order transition in the resistivity of the sintered pellets around 160K on cooling. The electronic properties including the transitional hysteresis in the resistance anomaly (from 80K-160K) are found to be very sensitive to the structural details of the samples, which were prepared in different annealing conditions. The thermopower results on the sintered pellets are reported between 10K - 300K. The magnetic measurements between 2K - 300K and up to 14 Tesla field show the absence of any magnetic ordering in Fe0.33VSe2. The magnetic moment per Fe -atom at room temperature (between 1.4 to 1.7 Bohr Magneton) is much lower than in previously reported anti-ferromagnetic FeV2Se4. Furthermore, the Curie constant shows a rapid and continuous reduction and combined with the high field magnetization result at 2K suggests a rapid decrease in the paramagnetic moments on cooling to low temperatures and the absence of any magnetic order in Fe0.33VSe2 at low temperatures.",0808.1334v1 2008-08-28,Giant frictional drag in strongly interacting bilayers near filling factor one,"We study the frictional drag in high mobility, strongly interacting GaAs bilayer hole systems in the vicinity of the filling factor $\nu=1$ quantum Hall state (QHS), at the same fillings where the bilayer resistivity displays a reentrant insulating phase. Our measurements reveal a very large longitudinal drag resistivity ($\rho^{D}_{xx}$) in this regime, exceeding 15 k$\Omega/\Box$ at filling factor $\nu=1.15$. $\rho^{D}_{xx}$ shows a weak temperature dependence and appears to saturate at a finite, large value at the lowest temperatures. Our observations are consistent with theoretical models positing a phase separation, e.g. puddles of $\nu=1$ QHS embedded in a different state, when the system makes a transition from the coherent $\nu=1$ QHS to the weakly coupled $\nu=2$ QHS.",0808.3807v1 2008-10-26,Development of Glass Resistive Plate Chambers for INO,"The India-based Neutrino Observatory (INO) collaboration is planning to build a massive 50kton magnetised Iron Calorimeter (ICAL) detector, to study atmospheric neutrinos and to make precision measurements of the parameters related to neutrino oscillations. Glass Resistive Plate Chambers (RPCs) of about 2m X 2m in size are going to be used as active elements for the ICAL detector. We have fabricated a large number of glass RPC prototypes of 1m X 1m in size and have studied their performance and long term stability. In the process, we have developed and produced a number of materials and components required for fabrication of RPCs. We have also designed and optimised a number of fabrication and quality control procedures for assembling the gas gaps. In this paper we will review our activities towards development of glass RPCs for the INO ICAL detector and will present results of the characterisation studies of the RPCs.",0810.4693v1 2009-02-01,"Enhancement of positive magnetoresistance following a magnetic-field-induced ferromagnetic transition in an intermetallic compound, Tb5Si3","We report the existence of a field-induced ferromagnetic transition in the magnetically ordered state (<69 K) of an intermetallic compound, Tb5Si3, and this transition is distinctly first-order at 1.8 K (near 60 kOe), whereas it appears to become second order near 20 K. The finding we stress is that the electrical resistivity becomes suddenly large in the high-field state after this transition and this is observed in the entire temperature range in the magnetically ordered state. Such an enhancement of 'positive' magnetoresistance (below 100 kOe) at the metamagnetic transition field is unexpected on the basis that the application of magnetic field should favor a low-resistive state due to alignment of spins.",0902.0153v1 2009-06-08,Tunneling Electroresistance in Ferroelectric Tunnel Junctions with a Composite Barrier,"Tunneling electroresistance (TER) effect is the change in the electrical resistance of a ferroelectric tunnel junction (FTJ) associated with polarization reversal in the ferroelectric barrier layer. Here we predict that a FTJ with a composite barrier that combines a functional ferroelectric film and a thin layer of a non-polar dielectric can exhibit a significantly enhanced TER. Due to the change in the electrostatic potential with polarization reversal the non-polar dielectric barrier acts as a switch that changes its barrier height from a low to high value. The predicted values of TER are giant and indicate that the resistance of the FTJ can be changed by many orders in magnitude at the coercive electric field of ferroelectric.",0906.1524v1 2009-08-11,Contrasting Pressure Effects in Sr2VFeAsO3 and Sr2ScFePO3,"We report the resistivity measurements under pressure of two Fe-based superconductors with a thick perovskite oxide layer, Sr2VFeAsO3 and Sr2ScFePO3. The superconducting transition temperature Tc of Sr2VFeAsO3 markedly increases with increasing pressure. Its onset value, which was Tc{onset}=36.4 K at ambient pressure, increases to Tc{onset}=46.0 K at ~4 GPa, ensuring the potential of the ""21113"" system as a high-Tc material. However, the superconductivity of Sr2ScFePO3 is strongly suppressed under pressure. The Tc{onset} of ~16 K decreases to ~5 K at ~4 GPa, and the zero-resistance state is almost lost. We discuss the factor that induces this contrasting pressure effect.",0908.1469v2 2010-03-11,Nonlinear response and two stable electrical conductivity levels measured in plasticized PVC thin film samples,"The electrical conductivity of PVC films prepared with a patented plasticizer of type ""A"" was measured with high precision automated setup, based on standard ring sell with a voltage range much less than breakdown voltage. Continual voltage-current measurements permit to take into account Debay relaxation process and clearly distinguish specific polymer film conductivity effects, connected with continuous current-stabilization behavior and transitions between two stable (long-living) states with several order magnitude different conductivities. Spontaneous reversible and non-destructive transitions of resistance levels was observed. For 30 mkm polymer films the values of sample resistance was measured equal to: high- 106 Ohm and low -103 Ohm.",1003.2331v1 2010-09-13,Non-monotonic temperature dependent transport in graphene grown by Chemical Vapor Deposition,"Temperature-dependent resistivity of graphene grown by chemical vapor deposition (CVD) is investigated. We observe in low mobility CVD graphene device a strong insulating behavior at low temperatures and a metallic behavior at high temperatures manifesting a non-monotonic in the temperature dependent resistivity.This feature is strongly affected by carrier density modulation. To understand this anomalous temperature dependence, we introduce thermal activation of charge carriers in electron-hole puddles induced by randomly distributed charged impurities. Observed temperature evolution of resistivity is then understood from the competition among thermal activation of charge carriers, temperature-dependent screening and phonon scattering effects. Our results imply that the transport property of transferred CVD-grown graphene is strongly influenced by the details of the environment",1009.2506v2 2010-10-14,Viscous corrections to the resistance of nano-junctions: a dispersion relation approach,"It is well known that the viscosity of a homogeneous electron liquid diverges in the limits of zero frequency and zero temperature. A nanojunction breaks translational invariance and necessarily cuts off this divergence. However, the estimate of the ensuing viscosity is far from trivial. Here, we propose an approach based on a Kramers-Kr\""onig dispersion relation, which connects the zero-frequency viscosity, $\eta(0)$, to the high-frequency shear modulus, $\mu_{\infty}$, of the electron liquid via $\eta(0) =\mu_{\infty} \tau$, with $\tau$ the junction-specific momentum relaxation time. By making use of a simple formula derived from time-dependent current-density functional theory we then estimate the many-body contributions to the resistance for an integrable junction potential and find that these viscous effects may be much larger than previously suggested for junctions of low conductance.",1010.2959v2 2011-05-18,Multiple photoexcitation of two-dimensional electron systems: bichromatic magnetoresistance oscillations revisited,"We analyze theoretically magnetoresistance of high mobility two-dimensional electron systems being illuminated by multiple radiation sources. In particular, we study the influence on the striking effect of microwave-induced resistance oscillations. We consider moderate radiation intensities without reaching the zero resistance states regime. We use the model of radiation-driven Larmor orbits extended to several light sources. First, we study the case of two different radiations polarized in the same direction with different or equal frequencies. For both cases we find a regime of superposition or interference of harmonic motions. When the frequencies are different, we obtain a modulated magnetoresistance response with pulses and beats. On the other hand, when the frequencies are the same, we find that the final result will depend on the phase difference between both radiation fields going from an enhanced response to a total collapse of oscillations, reaching an outcome similar to darkness. Finally, we consider a multiple photoexcitation case (three different frquencies) where we propose the two-dimensional electron system as a potential nanoantenna device for microwaves.",1105.3592v1 2011-07-11,Impairment of double exchange mechanism in electron transport of iron pnictides,"Double exchange mechanism is believed to favor transport along ferromagnetic directions, the failure of which in explaining the unusual resistivity anisotropy in iron pnictides is investigated. Several factors intrinsic to the microscopic mechanism of transport in iron pnictides are identified and analyzed, including the moderate Hund's coupling, low local moment, and presence of two anisotropic degenerate orbitals xz and yz. In particular, the substantial second neighbor hoppings are found to be decisive in giving results opposite to the double exchange picture. In high temperature nonmagnetic phase, orbital ordering is shown to give the right trend of resistivity anisotropy as observed experimentally, advocating its essential role in electron transport of iron pnictides.",1107.1952v1 2011-10-24,Anisotropy of upper critical fields and thermally-activated flux flow of quenched KxFe2-ySe2 single crystals,"We report the anisotropy of the upper critical fields mu0Hc2(T) and thermally-activated flux flow (TAFF) behavior of quenched KxFe2-ySe2. Even though the post-annealing and quenching process enhances the superconducting volume fraction, it has a minor effect on the upper critical fields for H//c and H//ab. Analysis of the angular-dependence of resistivity rho_ab(theta,H) indicates that it follows the scaling law based on the anisotropic Ginzburg-Landau (GL) theory and the anisotropy Gamma(T) increases with decreasing temperature with Gamma(T) ~ 3.6 at 27 K. The resistivity of quenched sample exhibits an Arrhenius TAFF behavior for both field directions. Field dependence of thermally activated energy U0(H) implies that the collective flux creep is dominant in high fields and point defects are the main pinning source in this regime.",1110.5316v1 2011-10-26,Mg substitution in CuCrO2 delafossite compounds,"A detailed investigation of the series CuCr(1-x)MgxO2 (x = 0.0 - 0.05) has been performed by making high-temperature resistivity and thermopower measurements, and by performing a theoretical analysis of the latter. Microstructure characterization has been carried out as well. Upon Mg2+ for Cr3+ substitution, a concomitant decrease in the electrical resistivity and thermopower values is found, up to x ~ 0.02 - 0.03, indicating a low solubility limit of Mg in the structure. This result is corroborated by scanning electron microscopy observations, showing the presence of MgCr2O4 spinels as soon as x = 0.005. The thermopower is discussed in the temperature-independent correlation functions ratio approximation as based on the Kubo formalism, and the dependence of the effective charge carrier density on the nominal Mg substitution rate is addressed. This leads to a solubility limit of 1.1% Mg in the delafossite, confirmed by energy dispersive X-ray spectroscopy analysis.",1110.5730v2 2011-11-09,Insulator-to-metal transition and large thermoelectric effect in La$_{1-x}$Sr$_{x}$MnAsO,"We report the Sr substitution effect in an antiferromagnetic insulator LaMnAsO. The Sr doping limit is $x\sim$ 0.10 under the synthesis conditions, as revealed by x-ray diffractions indicate. Upon Sr doping, the room-temperature resistivity drops by five orders of magnitude down to $\sim$0.01 $\Omega\cdot$cm, and the temperature dependence of resistivity shows essentially metallic behavior for $x\geq$0.08. Hall and Seebeck measurements confirm consistently that the insulator-to-metal transition is due to hole doping. Strikingly, the room-temperature Seebeck coefficient for the metallic samples is as high as $\sim240 \mu$V/K, making the system as a possible candidate for thermoelectric applications.",1111.2232v1 2011-11-23,Magneto-Electric Effects on Sr Z-type Hexaferrite at Room Temperature,"In this paper, magnetoelectric effects of Sr Z-type hexaferrite, Sr3Fe24Co2O41, at room temperature is measured. The change in remanence magnetization was measured by applying a DC voltage or electric field across a slab of hexaferrite. Changes of ~ 18% in remanence was observed in an electric field of 10,000V/cm implying a similar change in the microwave permeability at frequencies below 3GHz. Also, a change in dielectric constant at 1 GHz of ~16% in a magnetic field of only 320 Oe was measured. In these types of measurements high resistivity is critical in order to reduce current flow in the hexaferrite. The resistivity of the hexaferrite was raised to 4.28x10^8 ohm-cm by annealing under oxygen pressure. The measurements indicate that indeed electric polarization and magnetization changes were induced by the application of magnetic and electric fields, respectively. The implications for microwave applications appear to be very promising at room temperature.",1111.5555v1 2011-11-23,Room Temperature Magnetoelectric Effects on Single Slabs of Z-type Hexaferrites,"In this paper, magnetoelectric effects of Sr Z-type hexaferrite, Sr3Fe24Co2O41, at room temperature is measured. The change in remanence magnetization was measured by applying a DC voltage or electric field across a slab of hexaferrite. Changes of ~ 18% in remanence was observed in an electric field of 10,000V/cm implying a similar change in the microwave permeability at frequencies below 3GHz. In these types of measurements high resistivity is critical in order to reduce current flow in the hexaferrite. The resistivity of the hexaferrite was raised to 4.28x10^8 ohm?-cm by annealing under oxygen pressure. The measurements indicate that indeed electric polarization and magnetization changes were induced by the application of magnetic and electric fields, respectively. The implications for microwave applications appear to be very promising at room temperature.",1111.5556v1 2012-02-05,Temperature dependent elastic constants and ultimate strength of graphene and graphyne,"Based on the first principles calculation combined with quasi-harmonic approximation, in this work we focus on the analysis of temperature dependent lattice geometries, thermal expansion coefficients, elastic constants and ultimate strength of graphene and graphyne. For the linear thermal expansion coefficient, both graphene and graphyne show a negative region in the low temperature regime. This coefficient increases up to be positive at high temperatures. Graphene has superior mechanical properties, with Young modulus E11=371.0 N/m, E22=378.2 N/m and ultimate tensile strength of 119.2 GPa at room temperature. Based on our analysis, it is found that graphene's mechanical properties have strong resistance against temperature increase up to 1200 K. Graphyne also shows good mechanical properties, with Young modulus E11=224.7 N/m, E22=223.9 N/m and ultimate tensile strength of 81.2 GPa at room temperature, but graphyne's mechanical properties have a weaker resistance with respect to the increase of temperature than that of graphene.",1202.0933v1 2012-02-08,Coexisting Holes and Electrons in High-Tc Materials: Implications from Normal State Transport,"Normal state resistivity and Hall effect are shown to be successfully modeled by a two-band model of holes and electrons that is applied self-consistently to (i) DC transport data reported for eight bulk-crystal and six oriented-film specimens of YBa2Cu3O7-{\delta}, and (ii) far-infrared Hall angle data reported for YBa2Cu3O7-{\delta} and Bi2Sr2CaCu2O8+{\delta}. The electron band exhibits extremely strong scattering; the extrapolated DC residual resistivity of the electronic component is shown to be consistent with the previously observed excess thermal conductivity and excess electrodynamic conductivity at low temperature. Two-band hole-electron analysis of Hall angle data suggest that the electrons possess the greater effective mass.",1202.1792v1 2012-07-25,Superconductivity at 5.4 K in $β$-Bi$_2$Pd,"We investigate bulk superconductivity in a high-quality single crystal of Bi$_2$Pd ($\beta$-Bi$_2$Pd, space group; I4/mmm) at temperatures less than 5.4 K by exploring its electrical resistivity, magnetic susceptibility, and specific heat. The temperature dependence of the electrical resistivity shows convex-upward behaviors at temperatures greater than 40-50 K, which can be explained by a parallel-resistor model. In addition, we demonstrate that this material is a multiple-band/multiple-gap superconductor based on the temperature dependences of the specific heat and the upper critical field.",1207.5905v3 2012-10-09,Giant exchange bias and ferromagnetism in the CoO shell of Co/CoO-MgO core-shell nanoparticles,"Using magnetron sputtering, we produced a series of Co/CoO-MgO nanoparticles on Si(100) substrates. High-resolution transmission electron microscopy (HRTEM) image shows that small isolated Co-clusters (core) covered with CoO (shells) with a size of a few nm embedded in a MgO matrix. Resistivity as a function of Co atomic ratio exhibits a distinct percolation threshold with a sharp decrease around 69% Co content. Across the threshold, the resistivity drops about 7 orders of magnitude. For a sample at this percolation critical threshold, we have observed a giant exchange bias field HE=2460 Oe at T= 2K, and using soft x-ray magnetic circular dichroism at the Co-L2,3 edge, we have detected a ferromagnetic (FM) signal originating from the antiferromagnetic CoO shell. Moreover, decreasing the Mg-impurities will reduce the FM signal from CoO shell (namely the uncompensated spin density) and the size of HE, thus directly support the uncompensated spin model.",1210.2510v1 2012-11-12,Density dependent electrical conductivity in suspended graphene: Approaching the Dirac point in transport,"We theoretically consider, comparing with the existing experimental literature, the electrical conductivity of gated monolayer graphene as a function of carrier density, temperature, and disorder in order to assess the prospects of accessing the Dirac point using transport studies in high-quality suspended graphene. We show that the temperature dependence of graphene conductivity around the charge neutrality point provides information about how close the system can approach the Dirac point although competition between long-range and short-range disorder as well as between diffusive and ballistic transport may considerably complicate the picture. We also find that acoustic phonon scattering contribution to the graphene resistivity is always relevant at the Dirac point in contrast to higher density situations where the acoustic phonon contribution to the resistivity is strongly suppressed at the low temperature Bloch-Gr\""{u}neisen regime. We provide detailed numerical results for temperature and density dependent conductivity for suspended graphene.",1211.2845v2 2012-12-26,Molybdenum sputtering film characterization for high gradient accelerating structures,"Technological advancements are strongly required to fulfill the demands of new accelerator devices with the highest accelerating gradients and operation reliability for the future colliders. To this purpose an extensive R&D regarding molybdenum coatings on copper is in progress. In this contribution we describe chemical composition, deposition quality and resistivity properties of different molybdenum coatings obtained via sputtering. The deposited films are thick metallic disorder layers with different resistivity values above and below the molibdenum dioxide reference value. Chemical and electrical properties of these sputtered coatings have been characterized by Rutherford backscattering, XANES and photoemission spectroscopy. We will also present a three cells standing wave section coated by a molybdenum layer $\sim$ 500 nm thick designed to improve the performance of X-Band accelerating systems.",1212.6203v1 2012-12-28,Magneto-resistance up to 60 Tesla in Topological Insulator Bi2Te3 Thin Films,"We report magneto-transport studies of topological insulator Bi_{2}Te_{3} thin films grown by pulsed laser deposition. A non-saturating linear-like magneto-resistance (MR) is observed at low temperatures in the magnetic field range from a few Tesla up to 60 Tesla. We demonstrate that the strong linear-like MR at high field can be well understood as the weak antilocalization phenomena described by Hikami-Larkin-Nagaoka theory. Our analysis suggests that in our system, a topological insulator, the elastic scattering time can be longer than the spin-orbit scattering time. We briefly discuss our results in the context of Dirac Fermion physics and 'quantum linear magnetoresistance'.",1212.6464v1 2013-01-02,Visualizing Atomic-Scale Negative Differential Resistance in Bilayer Graphene,"We investigate the atomic-scale tunneling characteristics of bilayer graphene on silicon carbide using the scanning tunneling microscopy. The high-resolution tunneling spectroscopy reveals an unexpected negative differential resistance (NDR) at the Dirac energy, which spatially varies within the single unit cell of bilayer graphene. The origin of NDR is explained by two near-gap van Hove singularities emerging in the electronic spectrum of bilayer graphene under a transverse electric field, which are strongly localized on two sublattices in different layers. Furthermore, defects near the tunneling contact are found to strongly impact on NDR through the electron interference. Our result provides an atomic-level understanding of quantum tunneling in bilayer graphene, and constitutes a useful step towards graphene-based tunneling devices.",1301.0270v1 2013-04-01,Pressure Induced Superconductivity and Structural Transitions in Ba(Fe0.9Ru0.1)2As2,"High pressure electrical resistance and x-ray diffraction measurements have been performed on ruthenium-doped Ba(Fe0.9Ru0.1)2As2, up to pressures of 32 GPa and down to temperatures of 10 K, using designer diamond anvils under quasi-hydrostatic conditions. At 3.9 GPa, there is an evidence of pressure-induced superconductivity with Tc onset of 24 K and zero resistance at Tc zero of ~14.5 K. The superconducting transition temperature reaches maximum at ~5.5 GPa and then decreases gradually with increase in pressure before completely disappearing above 11.5 GPa. Upon increasing pressure at 200 K, an isostructural phase transition from a tetragonal (I4/mmm) phase to a collapsed tetragonal phase is observed at 14 GPa and the collapsed phase persists up to at least 30 GPa. The changes in the unit cell dimensions are highly anisotropic across the phase transition and are qualitatively similar to those observed in undoped BaFe2As2 parent.",1304.0298v2 2013-04-10,Charge Kondo Effect in Thermoelectric Properties of Lead Telluride doped with Thallium Impurities,"We investigate the thermoelectric properties of PbTe doped with a small concentration $x$ of Tl impurities acting as acceptors and described by Anderson impurities with negative on-site (effective) interaction. The resulting charge Kondo effect naturally accounts for a number of the low temperature anomalies in this system, including the unusual doping dependence of the carrier concentration, the Fermi level pinning and the self-compensation effect. The Kondo anomalies in the low temperature resistivity at temperatures $T\leq 10\, {\rm K}$ and the $x$-dependence of the residual resistivity are also in good agreement with experiment. Our model also captures the qualitative aspects of the thermopower at higher temperatures $T>300\, {\rm K}$ for high dopings ($x>0.6%$) where transport is expected to be largely dominated by carriers in the heavy hole band of PbTe.",1304.3026v1 2013-04-22,Modeling Composites of Multi-Walled Carbon Nanotubes in Polycarbonate,"High strain rate experiments performed on multi-walled carbon nanotubes and polycarbonate composites (MWCNT-PC) have exhibited enhanced impact resistance under a dynamic strain rate of nearly 2500/s with composition of only 0.5 to 2.0 percent of Multi walled carbon nanotubes(MWCNTs) in pure polycarbonate(PC). Similarly, hardness and elastic modulus under static loads resulted in significant increase depending upon the composition of MWCNTs in PC.The present work aims to analyze these results by correlating the data to fit expressions in generalizing the behavior of MWCNTs composition for MWCNT-PC composites under both static and impact loads. As a result we found that an optimum composition of 2.1 percent of MWCNTs exhibits maximum stress resistance within elastic range under strain rates of nearly 2500/s for MWCNT-PC composites.The results are critically dependent on the composition of MWCNTs and significantly deteriorate below and above a threshold composition. A simple model based on Lennard-Jones atom-atom based potential is formulated to compute static properties of pure as well as composites of PC.",1304.5979v1 2013-08-15,Suppression of bulk conductivity in InAs/GaSb broken gap composite quantum wells,"The two-dimensional topological insulator state in InAs/GaSb quantum wells manifests itself by topologically protected helical edge channel transport relying on an insulating bulk. This work investigates a way of suppressing bulk conductivity by using gallium source materials of different degrees of impurity concentrations. While highest-purity gallium is accompanied by clear conduction through the sample bulk, intentional impurity incorporation lead to a bulk resistance over 1 M\Omega. This resistance was found to be independent of applied magnetic fields. Ultra high electron mobilities for GaAs/AlGaAs structures fabricated in a molecular beam epitaxy system used for the growth of Sb-based samples are reported.",1308.3375v2 2013-09-06,Heteroepitaxy of Group IV-VI Nitrides by Atomic Layer Deposition,"Heteroepitaxial growth of selected group IV-VI nitrides on various orientations of sapphire (\alpha-Al2O3) is demonstrated using atomic layer deposition. High quality, epitaxial films are produced at significantly lower temperatures than required by conventional deposition methods. Characterization of electrical and superconducting properties of epitaxial films reveals a reduced room temperature resistivity and increased residual resistance ratio (RRR) for films deposited on sapphire compared to polycrystalline samples deposited concurrently on fused quartz substrates.",1309.1789v1 2013-10-31,Single crystal growth and characterization of the large-unit-cell compound Cu13Ba,"Single crystals of Cu$_{13}$Ba were successfully grown out of Ba-Cu self flux. Temperature dependent magnetization, $M(T)$, electrical resistivity, $\rho(T)$, and specific heat, $C_p(T)$, data are reported. Isothermal magnetization measurements, $M(H)$, show clear de Haas-van Alphen oscillations at $T$ = 2 K for applied fields as low as $\mu_0H$ = 1T. An anomalous behavior of the magnetic susceptibility is observed up to $T$ ~ 50K reflecting the effect of de Haas-van Alphen oscillations at fairly high temperatures. The field- and temperature-dependencies of the magnetization indicate the presence of diluted magnetic impurities with a concentration of the order of 0.01at.%. Accordingly, the minimum and lower temperature rise observed in the electrical resistivity at and below $T$ = 15K is attributed to the Kondo impurity effect.",1311.0027v1 2013-11-22,Thermally excited multi-band conduction in LaAlO3/SrTiO3 heterostructures exhibiting magnetic scattering,"Magnetotransport measurements of charge carriers at the interface of a LaAlO3/SrTiO3 heterostructure with 26 unit cells of LaAlO3 show Hall resistance and magnetoresistance which at low and high temperatures is described by a single channel of electron-like charge carriers. At intermediate temperatures, we observe non-linear Hall resistance and positive magnetoresistance, establishing the presence of at least two electron-like channels with significantly different mobilities and carrier concentrations. These channels are separated by 6 meV in energy and their temperature dependent occupation and mobilities are responsible for the observed transport properties of the interface. We observe that one of the channels has a mobility that decreases with decreasing temperature, consistent with magnetic scattering in this channel.",1311.5807v1 2014-04-18,Systematic control of carrier concentration and resisitivity in RF sputtered Zinc oxide thin films,"RF sputtered ZnO and Al:ZnO films are attractive transparent conductive oxides for fabrication of opto-electronic devices. In this paper we present efforts to control carrier concentration and mobility of ZnO/Al:ZnO thin films by controlling deposition parameters (RF power, pressure and substrate temperature. Al:ZnO thin film with resistivity as low as $\rho$ = $3.8\times 10^{-4}$ $\Omega$.cm at deposition temperature of 250{\deg}C has been achieved. Zinc oxide thin film with low resistivity of $\rho$ = $3.7\times 10^{-2}$ $\Omega$.cm and high electron mobility of $30$ $\mathrm{cm^{-2}V^{-1}s^{-1}}$ at deposition temperature of 250{\deg}C with acceptable electronic parameters stability has been obtained.Light transmission of Al:ZnO and ZnO samples deposited on glass at different substrate temperature has been studied. Investigation were made to assess the effect of deposition temperature on the photoluminescence spectra (PL) of ZnO/Al:ZnO sputtered on silicon and glass substrate. The evolution of near band edge (NBE) and deep level emission (DLE) photoluminescence peaks with deposition temperature in ZnO/Al:ZnO sputtered on Silicon and glass substrate have been studied.",1404.4902v1 2014-04-17,Caracterización de austenita expandida generada por cementación iónica de aceros inoxidables. Estudio de la estabilidad frente a la irradiación con haces de iones ligeros energéticos,"This thesis was focused on the surface modification with plasma discharge. Austenitic AISI 316L stainless steel sample was carburised under different experimental conditions and mechanical properties have been studied (thickness, lattice parameter, elemental composition, hardness, wear resistance and corrosion resistance). After that, steel substrates have been nitrided or carburised in order to analyse their stability under ion bombardment using a plasma focus device. Helium and deuterium were the gases used in 0, 1, 5, and 10 discharges. Optical and X-ray characterisations were used. Finally, using magnetron sputtering nitrided/carburised samples were coated with an AlN thin film in order to study their stability under long treatments at high temperatures.",1404.5204v1 2014-05-05,Controllable growth of Al nanorods for inexpensive and degradation-resistant surface enhanced Raman spectroscopy,"Surface enhanced Raman spectroscopy (SERS) has the capacity of detecting trace amount of biological or chemical matter, even single molecules, through the use of metallic nanostructures such as nanorods. Silver (Ag) and gold (Au) nanorods have led to the impressive enhancement of Raman signals, but they are either expensive, degrade fast over time, or suffer from poor sample repeatability. In contrast, Al is much less expensive, and Al nanorods could potentially be resistant to degradation over time due to the protection from native aluminum-oxide layers. Unfortunately, the controllable growth of Al nanorods has not been reported so far. This Letter reports, for the first time, the controllable growth of Al nanorods using physical vapor deposition (PVD); through the use of oxygen (O) surfactants. The enhancement factor of the Al nanorods in SERS is as high as 1250, and shows nearly no degradation after storage in ambient for 30 days or annealing at 475 K for one day.",1405.1009v1 2014-06-27,Simulation of Non-linear SRF losses derived from characteristic topography of etched and electropolished niobium surfaces,"A simplified numerical model has been developed to simulate non-linear superconducting radiofrequency (SRF) losses on Nb surfaces. This study focuses exclusively on excessive surface resistance (Rs) losses due to the microscopic topographical magnetic field enhancements. When the enhanced local surface magnetic field exceeds the superconducting critical transition magnetic field Hc, small volumes of surface material may become normal conducting and increase the effective surface resistance without inducing a quench. Using topographic data from typical Buffered Chemical Polish (BCP) and Electropolish (EP) treated fine grain niobium , we have estimated the resulting field-dependent losses and extrapolated this model to the implications for cavity performance. The model predictions correspond well to the characteristic BCP versus EP high field Q0 performance differences for fine grain niobium. We describe the algorithm of the model, its limitations, and the effects of this non-linear loss contribution on SRF cavity performance.",1406.7276v4 2015-01-25,Superconductivity in Dense Rashba Semiconductor BiTeCl,"Layered non-centrosymmetric bismuth tellurohalides are being examined as candidates for topological insulators. Pressure is believed to be essential for inducing and tuning topological order in these systems. Through electrical transport and Raman scattering measurements, we find superconductivity in two high-pressure phases of BiTeCl with the different normal state features, carrier characteristics, and upper critical field behaviors. Superconductivity emerges when the resistivity maximum or charge density wave is suppressed by the applied pressure and then persists till the highest pressure of 51 GPa measured. The huge enhancement of the resistivity with three magnitude of orders indicates the possible achievement of the topological order in the dense insulating phase. These findings not only enrich the superconducting family from topological insulators but also pave the road on the search of topological superconductivity in bismuth tellurohalides.",1501.06203v1 2015-02-04,Topological Insulator Thin Films Starting from the Amorphous Phase - Bi$_2$Se$_3$ as Example,"We present a new method to obtain topological insulator Bi$_2$Se$_3$ thin films with a centimeter large lateral length. To produce amorphous Bi$_2$Se$_3$ thin films we have used a sequential flash-evaporation method at room temperature. Transmission electron microscopy has been used to verify that the prepared samples are in a pure amorphous state. During annealing the samples transform into the rhombohedral Bi$_2$Se$_3$ crystalline strcuture which was confirmed using X-ray diffraction and Raman spectroscopy. Resistance measurements of the amorphous films show the expected Mott variable range hopping conduction process with a high specific resistance compared to the one obtained in the crystalline phase (metallic behavior). We have measured the magnetoresistance (MR) and the Hall effect (HE) at different temperatures between 2 K and 275 K. At temperatures $T \lesssim 50$ K and fields $B \lesssim 1$ T we observe weak anti-localization in the MR; the Hall measurements confirm the n-type character of the samples. All experimental results of our films are in quantitative agreement with results from samples prepared using more sophisticated methods.",1502.01135v1 2015-03-13,Suspended graphene devices with local gate control on an insulating substrate,"We present a fabrication process for graphene-based devices where a graphene monolayer is suspended above a local metallic gate placed in a trench. As an example we detail the fabrication steps of a graphene field-effect transistor. The devices are built on a bare high-resistivity silicon substrate. At temperatures of 77~K and below, we observe the field-effect modulation of the graphene resistivity by a voltage applied to the gate. This fabrication approach enables new experiments involving graphene-based superconducting qubits and nano-electromechanical resonators. The method is applicable to other two-dimensional materials.",1503.04147v2 2015-03-18,A novel fast timing micropattern gaseous detector: FTM,"In recent years important progress in micropattern gaseous detectors has been achieved in the use of resistive material to build compact spark-protected devices. The novel idea presented here consists of the polarisation of WELL structures using only resistive coating. This allows a new device to be built with an architecture based on a stack of several coupled layers where drift and WELL multiplication stages alternate in the structure. The signals from each multiplication stage can be read out from any external readout boards through the capacitive couplings. Each layer provides a signal with a gain of 10^4-10^5. The main advantage of this new device is the dramatic improvement of the timing provided by the competition of the ionisation processes in the different drift regions, which can be exploited for fast timing at the high luminosity accelerators (e.g. HL-LHC upgrade) as well as far applications like medical imaging.",1503.05330v1 2015-10-19,High resolution Hall measurements across the VO2 metal-insulator transition reveal impact of spatial phase separation,"Many strongly correlated transition metal oxides exhibit a metal-insulator transition (MIT), the manipulation of which is essential for their application as active device elements. However, such manipulation is hindered by lack of microscopic understanding of mechanisms involved in these transitions. A prototypical example is VO2, where previous studies indicated that the MIT resistance change correlate with changes in carrier density and mobility. We studied the MIT using Hall measurements with unprecedented resolution and accuracy, simultaneously with resistance measurements. Contrast to prior reports, we find that the MIT is not correlated with a change in mobility, but rather, is a macroscopic manifestation of the spatial phase separation which accompanies the MIT. Our results demonstrate that, surprisingly, properties of the nano-scale spatially-separated metallic and semiconducting domains actually retain their bulk properties. This study highlights the importance of taking into account local fluctuations and correlations when interpreting transport measurements in highly correlated systems.",1510.05414v1 2016-02-12,Relaxation of the resistive superconducting state in boron-doped diamond films,"We report a study of the relaxation time of the restoration of the resistive superconducting state in single crystalline boron-doped diamond using amplitude-modulated absorption of (sub-)THz radiation (AMAR). The films grown on an insulating diamond substrate have a low carrier density of about 2.5x10^{21} cm^{-3} and a critical temperature of about 2 K. By changing the modulation frequency we find a high-frequency rolloff which we associate with the characterstic time of energy relaxation between the electron and the phonon systems or the relaxation time for nonequilibrium superconductivity. Our main result is that the electron-phonon scattering time varies clearly as T^{-2}, over the accessible temperature range of 1.7 to 2.2 K. In addition, we find, upon approaching the critical temperature T_c, evidence for an increasing relaxation time on both sides of T_c.",1602.04046v1 2016-05-12,"Scalable, ultra-resistant structural colors based on network metamaterials","Structural colours have drawn wide attention for their potential as a future printing technology for various applications, ranging from biomimetic tissues to adaptive camouflage materials. However, an efficient approach to realise robust colours with a scalable fabrication technique is still lacking, hampering the realisation of practical applications with this platform. Here we develop a new approach based on large scale network metamaterials, which combine dealloyed subwavelength structures at the nanoscale with loss-less, ultra-thin dielectrics coatings. By using theory and experiments, we show how sub-wavelength dielectric coatings control a mechanism of resonant light coupling with epsilon-near-zero (ENZ) regions generated in the metallic network, manifesting the formation of highly saturated structural colours that cover a wide portion of the spectrum. Ellipsometry measurements report the efficient observation of these colours even at angles of $70$ degrees. The network-like architecture of these nanomaterials allows for high mechanical resistance, which is quantified in a series of nano-scratch tests. With such remarkable properties, these metastructures represent a robust design technology for real-world, large scale commercial applications.",1605.03700v1 2016-08-02,Low-energy electron-irradiation effect on transport properties of graphene field effect transistor,"We study the effects of low-energy electron beam irradiation up to 10 keV on graphene based field effect transistors. We fabricate metallic bilayer electrodes to contact mono- and bi-layer graphene flakes on SiO$_2$, obtaining specific contact resistivity $\rho_c \simeq 19 k\Omega \mu m^2$ and carrier mobility as high as 4000 cm$^2$V$^{-1}$s$^{-1}$. By using a highly doped p-Si/SiO$_2$ substrate as back gate, we analyze the transport properties of the device and the dependence on the pressure and on the electron bombardment. We demonstrate that low energy irradiation is detrimental on the transistor current capability, resulting in an increase of the contact resistance and a reduction of the carrier mobility even at electron doses as low as 30 $e^-/nm^2$. We also show that the irradiated devices recover by returning to their pristine state after few repeated electrical measurements.",1608.00716v1 2016-08-23,Disorder effect on the anisotropic resistivity of phosphorene determined by a tight-binding model,"In this work we develop a compact multi-orbital tight-binding model for phosphorene that accurately describes states near the main band gap. The model parameters are adjusted using as reference the band structure obtained by a density-functional theory calculation with the hybrid HSE06 functional. We use the optimized tight-binding model to study the effects of disorder on the anisotropic transport properties of phosphorene. In particular, we evaluate how the longitudinal resistivity depends on the lattice orientation for two typical disorder models: dilute scatterers with high potential fluctuation amplitudes, mimicking screened charges in the substrate, and dense scatterers with lower amplitudes, simulating weakly bounded adsorbates. We show that the intrinsic anisotropy associated to the band structure of this material, although sensitive to the type and intensity of the disorder, is robust.",1608.06633v2 2016-10-21,Giant Positive Magnetoresistance and field-induced metal insulator transition in Cr2NiGa,"We report here the magneto-transport properties of the newly synthesized Heusler compound Cr2NiGa which crystallizes in a disordered cubic B2 structure belonging to Pm-3m space group. The sample is found to be paramagnetic down to 2 K with metallic character. On application of magnetic field, a significantly large increase in resistivity is observed which corresponds to magnetoresistance as high as 112% at 150 kOe of field at the lowest temperature. Most remarkably, the sample shows negative temperature coefficient of resistivity below about 50 K under the application of field gretare than or equal to 80 kOe, signifying a field-induced metal to `insulating' transition. The observed magnetoresistance follows Kohler's rule below 20 K indicating the validity of the semiclassical model of electronic transport in metal with a single relaxation time. A multi-band model for electronic transport, originally proposed for semimetals, is found to be appropriate to describe the magneto-transport behavior of the sample.",1610.06771v1 2017-02-08,Hall field-induced resistance oscillations in MgZnO/ZnO heterostructures,"We report on nonlinear magnetotransport in a two-dimensional electron gas hosted in a MgZnO/ZnO heterostructure. Upon application of a direct current, we observe pronounced Hall field-induced resistance oscillations (HIRO) which are well known from experiments on high-mobility GaAs/AlGaAs quantum wells. The unique sensitivity of HIRO to the short-range component of the disorder potential allows us to unambiguously establish that the mobility of our MgZnO/ZnO heterostructure is limited by impurities residing within or near the 2D channel. Demonstration that HIRO can be realized in a system with a much lower mobility, much higher density, and much larger effective mass than in previously studied systems, highlights remarkable universality of the phenomenon and its great promise to be used in studies of a wide variety of emerging 2D materials.",1702.02557v1 2017-02-22,Variable-range-hopping conduction processes in oxygen deficient polycrystalline ZnO films,"We have fabricated oxygen deficient polycrystalline ZnO films by the rf sputtering deposition method. To systematically investigate the charge transport mechanisms in these samples, the electrical resistivities have been measured over a wide range of temperature from 300 K down to liquid-helium temperatures. We found that below about 100 K, the variable-range-hopping (VRH) conduction processes govern the charge transport properties. In particular, the Mott VRH conduction process dominates at higher temperatures, while crossing over to the Efros-Shklovskii (ES) VRH conduction process at lower temperatures. The crossover occurred at temperatures as high as a few tens degrees Kelvin. Moreover, the temperature behavior of resistivity over the entire VRH conduction regime from the Mott-type to the ES-type process can be well described by a universal scaling law.",1702.06729v1 2017-06-25,Coherent Interlayer Tunneling and Negative Differential Resistance with High Current Density in Double Bilayer Graphene-WSe2 Heterostructures,"We demonstrate gate-tunable resonant tunneling and negative differential resistance between two rotationally aligned bilayer graphene sheets separated by bilayer WSe2. We observe large interlayer current densities of 2 uA/um2 and 2.5 uA/um2, and peak-to-valley ratios approaching 4 and 6 at room temperature and 1.5 K, respectively, values that are comparable to epitaxially grown resonant tunneling heterostructures. An excellent agreement between theoretical calculations using a Lorentzian spectral function for the two-dimensional (2D) quasiparticle states, and the experimental data indicates that the interlayer current stems primarily from energy and in-plane momentum conserving 2D-2D tunneling, with minimal contributions from inelastic or non-momentum-conserving tunneling. We demonstrate narrow tunneling resonances with intrinsic half-widths of 4 and 6 meV at 1.5 K and 300 K, respectively.",1706.08034v1 2017-09-08,Coulomb drag and counterflow Seebeck coefficient in bilayer-graphene double layers,"We have fabricated bilayer-graphene double layers separated by a thin ($\sim$20 nm) boron nitride layer and performed Coulomb drag and counterflow thermoelectric transport measurements. The measured Coulomb drag resistivity is nearly three orders smaller in magnitude than the intralayer resistivities. The counterflow Seebeck coefficient is found to be well approximated by the difference between Seebeck coefficients of individual layers and exhibit a peak in the regime where two layers have opposite sign of charge carriers. The measured maximum counterflow power factor is $\sim$ 700 $\mu$W/K$^2$cm at room temperature, promising high power output per mass for lightweight thermoelectric applications. Our devices open a possibility for exploring the novel regime of thermoelectrics with tunable interactions between n-type and p-type channels based on graphene and other two-dimensional materials and their heterostructures.",1709.02778v1 2017-11-05,Synthesis of sodium cobaltate Na$_{x}$CoO$_{2}$ single crystals with controlled Na ordering,"In this study, we synthesized single crystals of Na$_{x}$CoO$_{2}$ with $x\sim0.8$ using the optical floating zone technique. A thorough electrochemical treatment of the samples permitted us to control the de-intercalation of Na to obtain single crystal samples of stable Na ordered phases with $x=0.5-0.8$. Comparisons of the bulk magnetic properties with those observed in the Na ordered powder samples confirmed the high quality of these single crystal phases. The ab plane resistivity was measured for the Na ordered samples and it was quite reproducible for different sample batches. The data were analogous to those found in previous initial experimental studies on single crystals, but the lower residual resistivity and sharper anti-ferromagnetic transitions determined for our samples confirmed their higher quality.",1711.01611v2 2018-01-19,Nontrivial Metallic State of Molybdenum Disulfide,"The electrical conductivity and Raman spectroscopy measurements have been performed on MoS$_2$ at high pressures up to 90 GPa and variable temperatures down to 5 K. We find that the temperature dependence of the resistance in a metallic 2H$_a$ phase has an anomaly (a hump) which shifts with pressure to higher temperature. Concomitantly, a new Raman phonon mode appears in the metallic state suggesting that the electrical resistance anomaly may be related to a structural transformation. We suggest that this anomalous behavior is due to a charge density wave state, the presence of which is indicative for a possibility for an emergence of superconductivity at higher pressures.",1801.06351v1 2019-05-23,Laser machined ultrathin microscale platinum thermometers on transparent oxide substrates,"Ultrathin microscale resistive thermometers are of key value to many applications. Here we have fabricated a laser machined 50 ${\mu}$m wide and 50 nm thick serpentine Pt thin film sensor capable of sensing temperatures up to 650 ${^\circ}$ C over multiple heating and cooling cycles. Various materials and associated processing conditions were studied, including both sapphire and silica as transparent substrates, alumina and TiO2 as adhesion layers, and lastly alumina and silicon oxide as capping layer. In-situ resistance monitoring helps to verify the multi-cycle stability of the sensor and guide the optimization. 10 ${\mu}$m sized sensors can be laser machined but will not survive multiple heating and cooling cycles. We demonstrate that the sensors with amorphous Ge thin layers can also repeatably measure temperatures up to 650 ${^\circ}$ C. It is anticipated that this sensor can be used for fast and high spatial resolution temperature probing for laser processing applications.",1905.09812v1 2014-08-06,Desarrollo de capas de AlN sobre aleaciones de aluminio como protección superficial contra la corrosión y el desgaste,"Aluminum and their alloys, after careful treatments, can develop excellent mechanical, tribological, electrical and chemical (high corrosion resistance) properties. However, 7000 series, with Cu in the alloy, have a poor corrosion resistance. On the other hand, aluminum nitride (AlN) has a wurtzitic phase and good thermal stability, optical, electric, piezoelectric, mechanical, tribological, and chemical properties, so the application range is huge. In this paper, AlN deposition on Al 7075 was done using the reactive magnetron sputtering technique in order to verify the aluminum nitride performance as an Al alloy protective film under wear and corrosive processes.",1408.1378v1 2014-08-28,Magneto-Dielectric Behavior in $La_{0.53}Ca_{0.47}MnO_{3}$,"We prospect magneto-dielectricity in $La_{0.53}Ca_{0.47}MnO_{3}$ across its paramagnetic (PMI) to ferromagnetic (FMM) isostructural transition at $T_{C} \sim 253K$, by magnetic ($(M)$), caloric ($(W)$), dielectric ($(\epsilon')$), magneto-resistive (MR), and magneto-capacitance (MC) investigations. Skew-broadened first-order transition character is confirmed via heating/cooling hystereses in $(M)(T)$ and $(W)(T)$, with superheating temperature $T**$ almost next to $T_C$ and supercooling temperature $T*$ exhibiting kinetics. Above $T_C$, linearly-related MC and MR reflect purely magneto-resistance effect. Near $T_C$, the high-frequency MC(5T) much exceeds the magneto-losses, and is uncorrelated with dc MR(5T) in the FM-ordered state. The intrinsic magneto-dielectricity manifest below $T_C$ and above ~kHz is traced to an intra-granular Maxwell-Wagner-type effect at the interface-region of PMI-FMM phase-coexistence.",1408.6640v2 2017-03-02,Thermal conduction across a boron nitride and silicon oxide interface,"The needs for efficient heat removal and superior thermal conduction in nano/micro devices have triggered tremendous studies in low-dimensional materials with high thermal conductivity. Hexagonal boron nitride (h-BN) is believed to be one of the candidates for thermal management and heat dissipation due to its novel physical properties, i.e. thermal conductor and electrical insulator. Here we reported interfacial thermal resistance between few-layer h-BN and its silicon oxide substrate using differential 3 omega method. The measured interfacial thermal resistance is around ~1.6*10-8 m2K/W for monolayer h-BN and ~3.4*10-8 m2K/W for 12.8nm-thick h-BN in metal/h-BN/SiO2 interfaces. Our results suggest that the voids and gaps between substrate and thick h-BN flakes limit the interfacial thermal conduction. This work provides a deeper understanding of utilizing h-BN flake as lateral heat spreader in electronic and optoelectronic nano/micro devices with further miniaturization and integration.",1703.00669v1 2019-02-10,The role of plastic strain gradients in the crack growth resistance of metals,"Crack advance from short or long pre-cracks is predicted by the progressive failure of a cohesive zone in a strain gradient, elasto-plastic solid. The presence of strain gradients leads to the existence of an elastic zone at the tip of a stationary crack, for both the long crack and the short crack cases. This is in sharp contrast with previous asymptotic analyses of gradient solids, where elastic strains were neglected. The presence of an elastic singularity at the crack tip generates stresses which are sufficiently high to activate quasi-cleavage. For the long crack case, crack growth resistance curves are predicted for a wide range of ratios of cohesive zone strength to yield strength. Remarkably, this feature of an elastic singularity is preserved for short cracks, leading to a severe reduction in tensile ductility. In qualitative terms, these predictions resemble those of discrete dislocation calculations, including the concept of a dislocation-free zone at the crack tip.",1902.03664v1 2019-07-11,Impurity concentration dependent electrical conduction in germanium crystal at low temperatures,"Germanium single crystal having 45 mm diameter and 100 mm length of 7N+ purity has been grown by Czochralski method. Structural quality of the crystal has been characterized by Laue diffraction. Electrical conduction and Hall measurements are carried out on samples retrieved from different parts of the crystal along the growth axis. Top part of the crystal exhibits lowest impurity concentration (~10^12/cm3) that gradually increases towards the bottom (10^13/cm3). The crystal is n-type at room temperature and the resistivity shows non-monotonic temperature dependence. There is a transition from n-type to p-type conductivity below room temperature at which bulk resistivity shows maximum and dip in carrier mobility. This intrinsic to extrinsic transition regions shift towards room temperature as the impurity concentration increases and reflects the purity level of the crystal. Similar trend is observed in boron implanted high purity germanium (HPGe) crystal at different doping level. The phenomena can be understood as a result of interplay between temperature dependent conduction mechanism driven by impurity band and intrinsic carrier in Ge crystals having fairly low acceptor concentrations (<10^12/cm3).",1907.05067v1 2020-02-25,Non-invasive nanoscale potentiometry and ballistic transport in epigraphene nanoribbons,"The recent observation of non-classical electron transport regimes in two-dimensional materials has called for new high-resolution non-invasive techniques to locally probe electronic properties. We introduce a novel hybrid scanning probe technique to map the local resistance and electrochemical potential with nm- and $\mu$V resolution, and we apply it to study epigraphene nanoribbons grown on the sidewalls of SiC substrate steps. Remarkably, the potential drop is non uniform along the ribbons, and $\mu$m-long segments show no potential variation with distance. The potential maps are in excellent agreement with measurements of the local resistance. This reveals ballistic transport in ambient condition, compatible with micrometer-long room-temperature electronic mean free paths.",2002.11024v1 2020-04-07,Multi-terminal electronic transport in boron nitride encapsulated TiS$_3$ nanosheets,"We have studied electrical transport as a function of carrier density, temperature and bias in multi-terminal devices consisting of hexagonal boron nitride (h-BN) encapsulated titanium trisulfide (TiS$_3$) sheets. Through the encapsulation with h-BN, we observe metallic behavior and high electron mobilities. Below $\sim$60 K an increase in the resistance, and non-linear transport with plateau-like features in the differential resistance are present, in line with the expected charge density wave (CDW) formation. Importantly, the critical temperature and the threshold field of the CDW phase can be controlled through the back-gate.",2004.03687v1 2020-04-09,Magnetic field-dependent resistance crossover and logarithmic to non-saturating magnetoresistance in topological insulator Bi$_2$Te$_3$,"We report a metal-insulator like transition in single crystalline 3D topological insulator Bi2Te3 at a temperature of 230K in presence of an external magnetic field applied normal to the surface. This transition becomes more prominent at larger magnetic field strength with the residual resistance value increasing linearly with the magnetic field. At low temperature, the magnetic field dependence of the magnetoresistance shows a transition from logarithmic to linear behavior and the onset magnetic field value for this transition decreases with increasing temperature. The logarithmic magnetoresistance indicates the weak anti-localization of the surface Dirac electrons while the high temperature behavior originates from the bulk carriers due to intrinsic impurities. At even higher temperatures beyond~230 K, a completely classical Lorentz model type quadratic behavior of the magnetoresistance is observed. We also show that the experimentally observed anomalies at ~230K in the magneto-transport properties do not originate from any stacking fault in Bi2Te3.",2004.04375v2 2012-01-02,Magnetodielectric behavior in La2CoMnO6 nanoparticles,"We have investigated magnetic, dielectric and magnetodielectric properties of La2CoMnO6 nanoparticles prepared by sol-gel method. Magnetization measurements revealed two distinct ferromagnetic transitions at 218 K and 135 K that can be assigned to ordered and disordered magnetic phases of the La2CoMnO6 nanoparticles. Two dielectric relaxations culminating around the magnetic transitions were observed with a maximum magnetodielectric response reaching 10% and 8% at the respective relaxation peaks measured at 100 kHz under 5T magnetic field. The dc electrical resistivity followed an insulating behavior and showed a negative magnetoresistance; there was no noticeable anomaly in resistivity or magnetoresistance near the magnetic ordering temperatures. Complex impedance analysis revealed a clear intrinsic contribution to the magnetodielectric response; however, extrinsic contribution due to Maxwell-Wagner effect combined with magnetoresistance property dominated the magnetodielectric effect at high temperatures.",1201.0448v1 2012-01-30,Unusual size effects on thermoelectricity in a strongly correlated oxide,"We investigated size effects on thermoelectricity in thin films of a strongly correlated layered cobaltate. At room temperature, the thermopower is independent of thickness down to 6 nm. This unusual behavior is inconsistent with the Fuchs-Sondheimer theory, which is used to describe conventional metals and semiconductors, and is attributed to the strong electron correlations in this material. Although the resistivity increases, as expected, below a critical thickness of $\sim$ 30 nm. The temperature dependent thermopower is similar for different thicknesses but resistivity shows systematic changes with thickness. Our experiments highlight the differences in thermoelectric behavior of strongly correlated and uncorrelated systems when subjected to finite size effects. We use the atomic limit Hubbard model at the high temperature limit to explain our observations. These findings provide new insights on decoupling electrical conductivity and thermopower in correlated systems.",1201.6274v1 2016-03-05,MIRO-like oscillations of magneto-resistivity in GaAs heterostructures induced by THz radiation,"We report on the study of terahertz radiation induced MIRO-like oscillations of magneto-resistivity in GaAs heterostructures. Our experiments provide an answer on two most intriguing questions - effect of radiation helicity and the role of the edges - yielding crucial information for understanding of the MIRO origin. Moreover, we demonstrate that the range of materials exhibiting radiation-induced magneto-oscillations can be largely extended by using high-frequency radiation.",1603.01760v1 2017-05-17,Epitaxial electrical contact to graphene on SiC,"Establishing good electrical contacts to nanoscale devices is a major issue for modern technology and contacting 2D materials is no exception to the rule. One-dimensional edge-contacts to graphene were recently shown to outperform surface contacts but the method remains difficult to scale up. We report a resist-free and scalable method to fabricate few graphene layers with electrical contacts in a single growth step. This method derives from the discovery reported here of the growth of few graphene layers on a metallic carbide by thermal annealing of a carbide forming metallic film on SiC in high vacuum. We exploit the combined effect of edge-contact and partially-covalent surface epitaxy between graphene and the metallic carbide to fabricate devices in which low contact-resistance and Josephson effect are observed. Implementing this approach could significantly simplify the realization of large-scale graphene circuits.",1705.08257v2 2017-07-10,Phonon-Driven Electron Scattering and Magnetothermoelectric Effect in Two-Dimensional Tin Selenide,"The bulk tin selenide (SnSe) is the best thermoelectric material currently with the highest figure-of-merit due to the strong phonon-phonon interactions. We investigate the effect of electron-phonon coupling (EPC) on the transport properties of two-dimensional (2D) SnSe sheet. We demonstrate that EPC plays a key role in the scattering rate where the constant relaxation time approximation is deficient. The EPC strength is especially large in contrast to that of pristine graphene. The scattering rate depends sensitively on the system temperatures and the carrier densities when the Fermi energy approaches the band edge. We also investigate the magnetothermoelectric effect of the 2D SnSe. It is found that at low temperatures there are enormous magnetoelectrical resistivity and magnetothermal resistivity above 500\%, suggesting the high potential for device applications. Our results agree reasonably well with the experimental data.",1707.02737v1 2019-03-05,Development of a time projection chamber with a sheet-resistor field cage,"A new-concept time projection chamber (TPC) using a commercial resistive sheet, sheet-resistor micro-TPC SR-microPIC, was developed and its performance was measured. SR-microTPC has the potential to create a more uniform electric field than conventional TPCs with resistor-chains owing to its continuous sheet resistivity, and its production would be easier than that of conventional TPCs. The material used in this study, Achilles-Vynilas, was found to be thin, transparent, and low-radioactive. The performance test with cosmic muons showed very promising results, including the demonstration of a good tracking-performance. This type of TPC field cage can offer an alternative for the widely used conventional field cages",1903.01663v3 2019-03-30,Disentangling spin-orbit coupling and local magnetism in a quasi-two-dimensional electron system,"Quantum interference between time-reversed electron paths in two dimensions leads to the well-known weak localization correction to resistance. If spin-orbit coupling is present, the resistance correction is negative, termed weak anti-localization (WAL). Here we report the observation of WAL coexisting with exchange coupling between itinerant electrons and localized magnetic moments. We use low-temperature magneto-transport measurements to investigate the quasi-two-dimensional, high-electron-density interface formed between SrTiO$_3$ (STO) and the anti-ferromagnetic Mott insulator NdTiO$_3$ (NTO). As the magnetic field angle is gradually tilted away from the sample normal, the data reveals the interplay between strong $k$-cubic Rashba-type spin-orbit coupling and a substantial magnetic exchange interaction from local magnetic regions. The resulting quantum corrections to the conduction are in excellent agreement with existing models and allow sensitive determination of the small magnetic moments (22 $\mu_B$ on average), their magnetic anisotropy and mutual coupling strength. This effect is expected to arise in other 2D magnetic materials systems.",1904.00295v2 2019-08-27,Large surface conductance and two-dimensional superconductivity in microstructured crystalline topological insulators,"Controllable geometric manipulation via micromachining techniques provides a promising tool for enhancing useful topological electrical responses relevant to future applications such as quantum information science. Here we present microdevices fabricated with focused ion beam from indium-doped topological insulator Pb1-xSnxTe. With device thickness on the order of 1 {\mu}m and an extremely large bulk resistivity, we achieve an unprecedented enhancement of the surface contribution to about 30% of the total conductance near room temperature. The surface contribution increases as the temperature is reduced, becoming dominant below approximately 180 K, compared to 30 K in mm-thickness crystals. In addition to the enhanced surface contribution to normal-state transport, we observe the emergence of a two-dimensional superconductivity below 6 K. Measurements of magnetoresistivity at high magnetic fields reveal a weak antilocalization behavior in the normal-state magnetoconductance at low temperature and a variation in the power-law dependence of resistivity on temperature with field. These results demonstrate that interesting electrical response relevant to practical applications can be achieved by suitable engineering of single crystals.",1908.10427v1 2019-12-11,Pressure-induced superconductivity and structural transition in ferromagnetic Cr2Si2Te6,"The discovery of intrinsic magnetism in atomically thin two-dimensional transition-metal trichalcogenides has attracted intense research interest due to the exotic properties of magnetism and potential applications in devices. Pressure has proven to be an effective tool to manipulate the crystal and electronic structures of the materials. Here, we report investigations on ferromagnetic van der Waals Cr2Si2Te6 via high-pressure synchrotron x-ray diffraction, electrical resistance, Hall resistance, and magnetoresistance measurements. Under compression, Cr2Si2Te6 simultaneously undergoes a structural transition, emergence of superconductivity at 3 K, sign change of the magnetoresistance, and dramatic change of the Hall coefficient at ~8 GPa. The superconductivity persists up to the highest measured pressure of 47.1 GPa with a maximum Tc = 4.5 K at ~30 GPa. The discovery of superconductivity in the two-dimensional van der Waals ferromagnetic Cr-based Cr2Si2Te6 provides new perspectives to explore superconductivity and the interplay between superconductivity and magnetism.",1912.05166v1 2012-06-23,Molecular-beam epitaxial growth of a far-infrared transparent electrode for extrinsic Germanium photoconductors,"We have evaluated the optical and electrical properties of a far-infrared (IR) transparent electrode for extrinsic germanium (Ge) photoconductors at 4 K, which was fabricated by molecular beam epitaxy (MBE). As a far-IR transparent electrode, an aluminum (Al)-doped Ge layer is formed at well-optimized doping concentration and layer thickness in terms of the three requirements: high far-IR transmittance, low resistivity, and excellent ohmic contact. The Al-doped Ge layer has the far-IR transmittance of >95 % within the wavelength range of 40--200 microns, while low resistivity (~5 ohm-cm) and ohmic contact are ensured at 4 K. We demonstrate the applicability of the MBE technology in fabricating the far-IR transparent electrode satisfying the above requirements.",1206.5368v1 2015-04-08,Post-growth purification of Co nanostructures prepared by focused electron beam induced deposition,"In the majority of cases nanostructures prepared by focused electron beam induced deposition (FEBID) employing an organometallic precursor contain predominantly carbon-based ligand dissociation products. This is unfortunate with regard to using this high-resolution direct-write approach for the preparation of nanostructures for various fields, such as mesoscopic physics, micromagnetism, electronic correlations, spin-dependent transport and numerous applications. Here we present an in-situ cleaning approach to obtain pure Co-FEBID nanostructures. The purification procedure lies in the exposure of heated samples to a H$_2$ atmosphere in conjunction with the irradiation by low-energy electrons. The key finding is that the combination of annealing at $300^\circ$C, H$_2$ exposure and electron irradiation leads to compact, carbon- and oxygen free Co layers down to a thickness of about 20\,nm starting from as-deposited Co-FEBID structures. In addition to this, in temperature-dependent electrical resistance measurements on post-processed samples we find a typical metallic behavior. In low-temperature magneto-resistance and Hall effect measurements we observe ferromagnetic behavior.",1504.01945v1 2015-06-22,"Preparation, characterization, and electrical properties of epitaxial NbO2 thin film lateral devices","Epitaxial NbO2 (110) films, 20 nm thick, were grown by pulsed laser deposition on Al2O3 (0001) substrates. The Ar/O2 total pressure during growth was varied to demonstrate the gradual transformation between NbO2 and Nb2O5 phases, which was verified using x-ray diffraction, x-ray photoelectron spectroscopy, and optical absorption measurements. Electric resistance threshold switching characteristics were studied in a lateral geometry using interdigitated Pt top electrodes in order to preserve the epitaxial crystalline quality of the films. Volatile and reversible transitions between high and low resistance states were observed in epitaxial NbO2 films, while irreversible transitions were found in case of Nb2O5 phase. Electric field pulsed current measurements confirmed thermally-induced threshold switching.",1506.06640v2 2018-07-25,Galvanomagnetic properties of the putative type-II Dirac semimetal PtTe$_2$,"Platinum ditelluride has recently been characterized, based on angle-resolved photoemission spectroscopy data and electronic band structure calculations, as a possible representative of type-II Dirac semimetals. Here, we report on the magnetotransport behavior (electrical resistivity, Hall effect) in this compound, investigated on high-quality single-crystalline specimens. The magnetoresistance (MR) of PtTe$_2$ is large (over $3000\%$ at $T=1.8$ K in $B=9$ T) and unsaturated in strong fields in the entire temperature range studied. The MR isotherms obey a Kohler's type scaling with the exponent $m$ = 1.69, different from the case of ideal electron-hole compensation. In applied magnetic fields, the resistivity shows a low-temperature plateau, characteristic of topological semimetals. In strong fields, well-resolved Shubnikov - de Haas (SdH) oscillations with two principle frequencies were found, and their analysis yielded charge mobilities of the order of $10^3\,\rm{cm^2V^{-1}s^{-1}}$ and rather small effective masses of charge carriers, $0.11m_e$ and $0.21m_e$. However, the extracted Berry phases point to trivial character of the electronic bands involved in the SdH oscillations. The Hall effect data corroborated a multi-band character of the electrical conductivity in PtTe$_2$, with moderate charge compensation.",1807.09876v1 2018-12-18,An application of extensions of the Ramo-Shockley theorem to signals in silicon sensors,"We discuss an extension of the Ramo-Shockley theorem that allows the calculation of signals in detectors that contain non-linear materials of arbitrary permittivity and finite conductivity (volume resistivity) as well as a static space-charge. The readout-electrodes can be connected by an arbitrary impedance network. This formulation is useful for the treatment of semiconductor sensors where the finite volume resistivity in the sensitive detector volume cannot be neglected. The signals are calculated by means of time dependent weighting fields and weighting vectors. These are calculated by adding voltage or current signals to the electrodes in question, which has a very practical application when using semiconductor device simulation programs. An analytic example for an un-depleted silicon sensor is given.",1812.07570v2 2018-12-19,"Blue (In,Ga)N Light-Emitting Diodes with Buried n+-p+ Tunnel Junctions by Plasma-Assisted Molecular Beam Epitaxy","Blue light-emitting diodes (LEDs) consisting of a buried n+-p+ GaN tunnel junction, (In,Ga)N multiple quantum wells (MQWs) and a n+-GaN top layer are grown on single-crystal Ga-polar n+-GaN bulk wafers by plasma-assisted molecular beam epitaxy. The (In,Ga)N MQW active regions overgrown on the p+-GaN show chemically abrupt and sharp interfaces in a wide range of compositions and are seen to have high structural and optical properties as verified by X-ray diffraction and spatially resolved cathodoluminescence measurements. The processed LEDs reveal clear rectifying behavior with a low contact and buried tunnel junction resistivity. By virtue of the top n+-GaN layer with a low resistance, excellent current spreading in the LEDs is observed at low currents in this device structure. A few of new device possibilities based on this unique design are discussed.",1812.07708v1 2019-01-07,Growth and Characterization of Fe0.95Se0.6Te0.4 Single Crystal,"In this paper we present the single crystal growth of Fe0.95Se0.6Te0.4 high TC superconducting sample by the modified Bridgman technique. The x-ray diffraction pattern shows the single crystal nature of the sample, as only (00l) peaks are detectable. The stoichiometric composition has been verified by energy dispersive x-ray analysis. The superconducting transition temperature at 14 K was confirmed through DC magnetization (ZFC-FC) and resistivity measurements. By analyzing the isothermal M-H curves, we determined the value of H_c1 (0) ~360 Oe by extrapolating the data. The temperature coefficient of resistivity obtained using the power law fitting was found to be 0.6. The obtained Raman spectra at room temperature can be interpreted with the tetragonal crystal structure and space group P4/nmm.",1901.01955v1 2019-11-06,Low frequency imaginary impedance at the superconducting transition of 2H-NbSe$_2$,"The superconducting transition leads to a sharp resistance drop in a temperature interval that can be a small fraction of the critical temperature T$_c$. A superconductor exactly at T$_c$ is thus very sensitive to all kinds of thermal perturbations, including the heat dissipated by the measurement current. We show that the interaction between electrical and thermal currents leads to a sizeable imaginary impedance at frequencies of order of tens of Hz at the resistive transition of single crystals of the layered material 2H-NbSe$_2$. We explain the result using models developed for transition edge sensors. By measuring under magnetic fields and at high currents, we find that the imaginary impedance is strongly influenced by the heat associated with vortex motion and out-of-equilibrium quasiparticles.",1911.02340v2 2020-01-15,Enhanced Carrier Transport by Transition Metal Doping in WS2 Field Effect Transistors,"High contact resistance is one of the primary concerns for electronic device applications of two-dimensional (2D) layered semiconductors. Here, we explore the enhanced carrier transport through metal-semiconductor interfaces in WS2 field effect transistors (FETs) by introducing a typical transition metal, Cu, with two different doping strategies: (i) a ""generalized"" Cu doping by using randomly distributed Cu atoms along the channel and (ii) a ""localized"" Cu doping by adapting an ultrathin Cu layer at the metal-semiconductor interface. Compared to the pristine WS2 FETs, both the generalized Cu atomic dopant and localized Cu contact decoration can provide a Schottky-to-Ohmic contact transition owing to the reduced contact resistances by 1 - 3 orders of magnitude, and consequently elevate electron mobilities by 5 - 7 times higher. Our work demonstrates that the introduction of transition metal can be an efficient and reliable technique to enhance the carrier transport and device performance in 2D TMD FETs.",2001.05105v1 2020-01-20,Electrical conduction mechanisms of metal / high-Tc superconductor (YBCO) interfaces,"Current-voltage characteristics of Au~/~YBa$_2$Cu$_3$O$_{7-\delta}$ interfaces (Au/YBCO), built on optimally-doped YBCO thin films, grown by pulsed laser deposition, were measured as a function of temperature in the 50 K to 270 K range, for two different resistance states. A non-trivial equivalent circuit model is proposed, which reveals the existence of a highly inhomogeneous scenario composed by two complex layers: one presenting both a non-linear Poole-Frenkel conduction as well as Variable Range Hopping localization effects (probably associated with YBa$_2$Cu$_3$O$_{6}$) mixed with a minor metallic phase, while the other is also composed by a mixture of YBCO with different oxygen contents, where a metallic ohmic phase still percolates. A microscopic description of the effects produced by the resistance switching is given, showing the evolution of carrier traps, localization effects and dielectric behavior for each state. The dielectric behavior is interpreted in terms of a Maxwell-Wagner scenario.",2001.07237v1 2020-06-09,Fluctuations superconductivity and giant negative magnetoresistance in a gate voltage tuned 2D electron liquid with strong spin-orbit impurity scattering,"We present a quantitative theory of the gate-voltage tuned superconductor-to-insulator transition (SIT) observed experimentally in the 2D electron liquid created in the (111) interface between crystalline SrTiO_3 and LaAlO_3 . Considering two fundamental opposing effects of Cooper-pair fluctuations; the critical conductivity enhancement, known as para-conductivity, and its suppression associated with the loss of unpaired electrons due to Cooper-pairs formation, we employ the standard thermal fluctuations theory, modified to include quantum fluctuations within a novel phenomenological approach. Relying on the quantitative agreement found between our theory and a large body of experimental sheet-resistance data, we conclude that spin-orbit scatterings, via significant enhancement of the interaction between fluctuations, strongly enhance the sheet resistance peak at high fields, and reveal anomalous metallic behavior at low fields, due to mixing of relatively heavy electron bands with a light electron band near a Lifshitz point.",2006.05098v3 2020-08-15,Ultrahigh Doping of Graphene Using Flame-Deposited MoO3,"The expected high performance of graphene-based electronics is often hindered by lack of adequate doping, which causes low carrier density and large sheet resistance. Many reported graphene doping schemes also suffer from instability or incompatibility with existing semiconductor processing. Here we report ultrahigh and stable p-type doping up to ~7x10^13 1/cm^2 (~2x10^21 1/cm^3}) of monolayer graphene grown by chemical vapor deposition. This is achieved by direct polycrystalline MoO3 growth on graphene using a rapid flame synthesis technique. With this approach, the metal-graphene contact resistance for holes is reduced to ~200 Ohm-um. We also demonstrate that flame-deposited MoO3 provides over 5x higher doping of graphene, as well as superior thermal and long-term stability, compared to electron-beam deposited MoO3.",2008.06794v1 2020-11-13,Large anomalous Hall angle in a topological semimetal candidate TbPtBi,"The magnetotransport properties in antiferromagnetic half-Heusler single crystals of TbPtBi, a magnetic-field-induced topological semimetal with simple band structure, are investigated. We found that a nonmonotonic magnetic field dependence of the anomalous Hall resistivity in a high magnetic field (B>7T), which come from the change of band structure induced by the Zeeman-like splitting when applying the external magnetic field. The experiment results show that credible anomalous Hall resistivity and conductivity reach up to 0.6798m{\Omega}cm and 125{\Omega}-1cm-1, respectively. A large AHA up to 33% is obtained in TbPtBi, which is comparable to typical ferromagnetic Weyl semimetal. The analysis of results show it should be attributed to topological band around EF and low carrier density.",2011.06864v1 2021-03-09,Anisotropy of the In-Plane and Out-of-Plane Resistivity and the Hall Effect in the Normal State of Vicinal-Grown YBa$_{2}$Cu$_{3}$O$_{7-δ}$ Thin Films,"The resistivity and the Hall effect in the copper-oxide high-temperature superconductor YBa$_{2}$Cu$_{3}$O$_{7-\delta}$ (YBCO) are remarkably anisotropic. Using a thin film of YBCO grown on an off-axis cut SrTiO$_3$ substrate allows one to investigate these anisotropic transport properties in a planar and well-defined sample geometry employing a homogeneous current density. In the normal state, the Hall voltage probed parallel to the copper-oxide layers is positive and strongly temperature dependent, whereas the out-of-plane Hall voltage is negative and almost temperature independent. The results confirm previous measurements on single crystals by an entirely different measurement method and demonstrate that vicinal thin films might be also useful for investigations of other layered nanomaterials.",2103.05511v1 2021-06-24,Erasable superconductivity in topological insulator Bi2Se3 induced by voltage pulse,"Three-dimensional topological insulators (TIs) attract much attention due to its topologically protected Dirac surface states. Doping into TIs or their proximity with normal superconductors can promote the realization of topological superconductivity(SC) and Majorana fermions with potential applications in quantum computations. Here, an emergent superconductivity was observed in local mesoscopic point-contacts on the topological insulator Bi2Se3 by applying a voltage pulse through the contacts, evidenced by the Andreev reflection peak in the point-contact spectra and a visible resistance drop in the four-probe electrical resistance measurements. More intriguingly, the superconductivity can be erased with thermal cycles by warming up to high temperatures (300 K) and induced again by the voltage pulse at the base temperature (1.9 K), suggesting a significance for designing new types of quantum devices. Nematic behaviour is also observed in the superconducting state, similar to the case of CuxBi2Se3 as topological superconductor candidates.",2106.13207v1 2021-06-29,Low Resistance III-V Hetero-contacts to N-Ge,"We experimentally study III-V/Ge heterostructure and demonstrate InGaAs hetero-contacts to n-Ge with a wide range of In % and achieve low contact resistivity ($\rho_C$) of $5\times10^{-8} \Omega\cdot cm^2$ for Ge doping of $3 \times 10^{19} cm^{-3}$. This results from re-directing the charge neutrality level (CNL) near the conduction band and benefiting from low effective mass for high electron transmission. For the first time, we observe that the heterointerface presents no temperature dependence despite the two different conduction minimum valley locations of III-V ($\Gamma$-valley) and Ge (L-valley), which potentially stems from elastic trap-assisted tunneling through defect states at the interface generated by dislocations. The hetero-interface plays a dominant role in the overall $\rho_C$ below $\approx 1 \times 10^{-7} \Omega \cdot cm^2$, which can be further improved with large active dopant concentration in Ge by co-doping.",2106.15099v1 2021-09-08,Unusual Magnetic Properties in Layered Magnetic Topological Insulator EuSn2As2,"EuSn2As2 with layered rhombohedral crystal structure is proposed to be a candidate of intrinsic antiferromagnetic (AFM) topological insulator. Here, we have investigated systematic magnetoresistance (MR) and magnetization measurements on the high quality EuSn2As2 single crystal with the magnetic field both parallel and perpendicular to (00l) plane. Both the kink of magnetic susceptibility and longitudinal resistivity reveal that EuSn2An2 undergoes an AFM transition at TN = 21 K. At T = 2 K, the magnetization exhibits two successive plateaus of ~ 5.6 {\mu}B/Eu and ~ 6.6 {\mu}B/Eu at the corresponding critical magnetic fields. Combined with the negative longitudinal MR and abnormal Hall resistance, we demonstrate that EuSn2An2 undergoes complicated magnetic transitions from an AFM state to a canted ferromagnetic (FM) state at Hc and then to a polarized FM state at Hs as the magnetic field increase.",2109.03414v1 2022-05-12,Shubnikov-de Haas and de Haas-van Alphen oscillation in Czochralski grown CoSi single crystal,"Anisotropic transport, Shubnikov-de Haas (SdH), and de Haas-van Alphen (dHvA) quantum oscillations studies are reported on a high-quality CoSi single crystal grown by the Czochralski method. Temperature-dependent resistivities indicate the dominating electron-electron scattering. Magnetoresistance (MR) at 2 K reaches 610% for I||[111] and B||[01-1], whereas it is 500% for I||[01-1] and B||[111]. A negative slope in field-dependent Hall resistivity suggests electrons are the majority carriers. The carrier concentration extracted from Hall conductivity indicates no electron-hole compensation. In 3D CoSi, the electron transport lifetime is found to be approximately in the same order as quantum lifetime, whereas in 2D electron gas the long-range scattering drives the transport life much larger than the quantum lifetime. From linear and Hall SdH oscillations the effective masses and Dingle temperatures have been calculated. The dHvA oscillation reveals three frequencies at 18 ($\gamma$), 558 ($\alpha$) and 663 T ($\beta$)), whereas, SdH oscillation results in only two frequencies $\alpha$ and $\beta$. The $\gamma$ frequency observed in dHvA oscillation is a tiny hole pocket at the $\Gamma$ point.",2205.05881v1 2022-07-05,Anderson localization crossover in 2D Si systems: The past and the present,"Using Ioffe-Regel-Mott (IRM) criterion for strong localization crossover in disordered doped 2D electron systems, we theoretically study the relationships among the three key experimentally determined localization quantities: critical density ($n_\mathrm{c}$), critical resistance ($\rho_\mathrm{c}$), and sample quality defined by the effective impurity density (as experimentally diagnosed by the sample mobility, $\mu_\mathrm{m}$, at densities much higher than critical densities). Our results unify experimental results for 2D metal-insulator transitions (MIT) in Si systems over a 50-year period (1970-2020), showing that $n_\mathrm{c}$ ($\rho_\mathrm{c}$) decrease (increase) with increasing sample quality, explaining why the early experiments in the 1970s, using low-quality samples ($\mu_\mathrm{m} \sim 10^3 \mathrm{cm}^2/Vs$) reported strong localization crossover at $n_c \sim 10^{12} \mathrm{cm}^{-2}$ with $\rho_c \sim 10^3\Omega$ whereas recent experiments (after 1995), using high-quality samples ($\mu_\mathrm{m} >10^4 \mathrm{cm}^2/Vs$), report $n_c \sim 10^{11} \mathrm{cm}^{-2}$ with $\rho_c>10^4\Omega$. Our theory establishes the 2D MIT to be primarily a screened Coulomb disorder-driven strong localization crossover phenomenon, which happens at different sample-dependent critical density and critical resistance, thus unifying Si 2D MIT phenomena over a 50-year period.",2207.02220v1 2022-08-22,Electronic structure and physical properties of EuAuAs single crystal,"High-quality single crystals of EuAuAs were studied by means of powder x-ray diffraction, magnetization, magnetic susceptibility, heat capacity, electrical resistivity and magnetoresistance measurements. The compound crystallizes with a hexagonal structure of the ZrSiBe type (space group $P6_3/mmc$). It orders antiferromagnetically below 6 K due to the magnetic moments of divalent Eu ions. The electrical resistivity exhibits metallic behavior down to 40 K, followed by a sharp increase at low temperatures. The magnetotransport isotherms show a distinct metamagnetic-like transition in concert with the magnetization data. The antiferromagnetic ground state in \mbox{EuAuAs} was corroborated in the \textit{ab initio} electronic band structure calculations. Most remarkably, the calculations revealed the presence of nodal line without spin-orbit coupling and Dirac point with inclusion of spin-orbit coupling. The \textit{Z}$_2$ invariants under the effective time reversal and inversion symmetries make this system nontrivial topological material. Our findings, combined with experimental analysis, makes EuAuAs a plausible candidate for an antiferromagnetic topological nodal-line semimetal.",2208.10405v1 2022-09-18,Superparamagnetic and metal-like Ru2TiGe: a propitious thermoelectric material,"We report a study of structural, magnetic, heat capacity and thermoelectric properties of a Rubased Heusler alloy, Ru2TiGe. The magnetic measurements reveal that at higher temperatures, diamagnetic and Pauli paramagnetic contributions dominate the magnetic behaviour whereas, at lower temperatures (T<= 20 K), superparamagnetic interaction among clusters is observed. Effect of such magnetic defects is also evident in the electrical resistivity behaviour at lower temperatures. Though the temperature dependence of resistivity exhibits a metal-like nature, the large value of Seebeck coefficient leads to an appreciable power factor of the order of 1 mW/mK2 at 300 K. Large power factor as well as low thermal conductivity results in a value of ZT = 0.025 at 390 K for Ru2TiGe that is orders of magnitude higher than that of the other pure Heusler alloys and point towards its high potential for practical thermoelectric applications.",2209.08474v1 2022-11-02,Umklapp electron-electron scattering in bilayer graphene moiré superlattice,"Recent experimental advances have been marked by the observations of ballistic electron transport in moir\'e superlattices in highly aligned heterostructures of graphene and hexagonal boron nitride (hBN). Here, we predict that a high-quality graphene bilayer aligned with an hBN substrate features $T^2$-dependent resistivity caused by umklapp electron-electron (Uee) scattering from the moir\'e superlattice, that is, a momentum kick by Bragg scattering experienced by a pair of electrons. Substantial Uee scattering appears upon $p$-doping of the bilayer above a threshold density, which depends on the twist angle between graphene and hBN, and its contribution towards the resistivity grows rapidly with hole density until it reaches a peak value, whose amplitude changes non-monotonically with the superlattice period. We also analyse the influence of an electrostatically induced bandgap in the bilayer and trigonal warping it enhances in the electron dispersion on the electron-electron umklapp scattering.",2211.01005v1 2023-01-11,Application of the partial Dirichlet-Neumann contact algorithm to simulate low-velocity impact events on composite structures,"Impact simulations for damage resistance analysis are computationally intensive due to contact algorithms and advanced damage models. Both methods, which are the main ingredients in an impact event, require refined meshes at the contact zone to obtain accurate predictions of the contact force and damage onset and propagation through the material. This work presents the application of the partial Dirichlet-Neumann contact algorithm to simulate low-velocity impact problems on composite structures using High-Performance Computing. This algorithm is devised for parallel finite element codes running on supercomputers, and it is extended to explicit time integration schemes to solve impact problems including damage. The proposed framework is validated with a standard test for damage resistance on fiber-reinforced polymer matrix composites. Moreover, the parallel performance of the proposed algorithm has been evaluated in a mesh of 74M of elements running with 2400 processors.",2301.05552v2 2023-01-19,Unusual anisotropic magnetoresistance due to magnetization-dependent spin-orbit interactions,"One of recent surprising discoveries is the unusual anisotropic magnetoresistance (UAMR) that depends on two magnetization components perpendicular to the current differently, in contrast to the conventional anisotropic magnetoresistance (AMR) that predicts no change in resistance when the magnetization varies in the plane perpendicular to the current. Using density functional theory and Boltzmann transport equation calculations for bcc Fe, hcp Co, and bcc FeCo alloys, we show that UAMR can be accounted by the magnetization-dependent spin-orbit interactions (SOI): Magnetization-dependent SOI modifies electron energy bands that, in turn, changes resistance. A phenomenological model reveals the intrinsic connection between SOI and order-parameters. Such a mechanism is confirmed by the strong biaxial stain effect on UAMR. Our findings provide an efficient way of searching and optimizing materials with large UAMR, important in the design of high-performance spintronic devices.",2301.07886v1 2023-03-06,Timing resistive plate chambers for thermal neutron detection with 3D position sensitivity,"An optimized design of a neutron detector based on timing RPCs (Resistive Plate Chambers) with boron-10 neutron converters is presented. The detector is composed of a stack of ten double gap RPCs with aluminium cathode plates coated on both sides with $^{10}B_{4}C$. This design enables simultaneous determination with high accuracy of both the neutron time-of-flight (down to ns resolution) and the interaction position in 3D (down to 0.25 mm resolution across and ~1 mm along the beam). It is shown that the detection efficiency can approach 60% for neutrons with $\lambda$ = 4.7 \.A. A new geometry with less material budget is introduced for the signal pick-up strip arrays. The results of simulation-based optimization of the design are reported considering the trade-off between the detection efficiency, the count rate capability and the amount of elastic scattering on the detector components.",2303.03461v1 2023-03-22,Effect of gamma radiation on electrical properties of diffusive memristor devices,"Diffusive memristors continue to receive tremendous interest due to their ability to emulate biological neurons and thus aid the development of bio-inspired computation technology. A major issue with the diffusive memristor is the inability to reliably control the formation of the conduction filaments which affects both the device functionality and reproducibility of regimes after each application of voltage. Here we investigate the effect of gamma radiation on the electrical properties of the diffusive memristors based on metallic nanoparticles in dielectric matrix. Our experiments show that after exposing to radiation, the memristors demonstrate much sharper (and less noisy) hysteresis in the current-voltage characteristics while preserving the same low- and high-resistive states as in the pristine samples. Additionally, the radiation lowers both threshold and hold voltages that correspond to onset of low- and high- resistive states, respectively. The proposed mechanism involves radiation-induced defects in the silica matrix which help to establish dominant pathways for nanoparticles to form conduction filaments. Our findings suggest an efficient way to enhance working characteristics of diffusive memristors and to improve their reproducibility.",2303.12762v1 2023-07-18,Universal scaling near band-tuned metal-insulator phase transitions,"We present a theory for band-tuned metal-insulator transitions based on the Kubo formalism. Such a transition exhibits scaling of the resistivity curves, in the regime where $T\tau >1$ or $\mu \tau>1$, where $\tau$ is the scattering time and $\mu$ the chemical potential. At the critical value of the chemical potential, the resistivity diverges as a power law, $R_c \sim 1/T$. Consequently, on the metallic side there is a regime with negative $dR/dT$, which is often misinterpreted as insulating. We show that scaling and this `fake insulator' regime is observed in a wide range of experimental systems. In particular, we show that Mooij correlations in high-temperature metals with negative $dR/dT$ can be quantitatively understood with our scaling theory in the presence of $T$-linear scattering.",2307.09292v1 2023-10-10,The black hole to black hole phase transition probed by the D3-D7 model fermionic spectral functions,"We consider the D3-D7 model and analyze the phase transition from the black-hole phase to another black-hole phase using the spectral function of a probe fermion on D7 in the presence of the finite density and temperature. From the fermionic spectral functions, we study the temperature dependence of the decay rate and we observe a jump in it at the critical temperature that corresponds to the first order phase transition. We found that if we assume that the Drude model works in this case so that the resistivity is proportional to the fermion decay rate, the jump matches the resistivity data in a heavy fermion material.",2310.06317v1 2023-10-22,Electrical conductivity enhancement of epitaxially grown TiN thin films,"Titanium nitride (TiN) presents superior electrical conductivity with mechanical and chemical stability and compatibility with the semiconductor fabrication process. Here, we fabricated epitaxial and polycrystalline TiN (111) thin films on MgO (111), sapphire (001), and mica substrates at 640oC and room temperature by using a DC sputtering, respectively. The epitaxial films show less amount of surface oxidation than the polycrystalline ones grown at room temperature. The epitaxial films show drastically reduced resistivity (~30 micro-ohm-cm), much smaller than the polycrystalline films. Temperature-dependent resistivity measurements show a nearly monotonic temperature slope down to low temperature. These results demonstrate that high temperature growth of TiN thin films leads to significant enhancement of electrical conductivity, promising for durable and scalable electrode applications.",2310.14208v1 2023-11-20,Magnetic-field-induced nonlinear transport in HfTe5,"The interplay of electron correlations and topological phases gives rise to various exotic phenomena including fractionalization, excitonic instability, and axionic excitation. Recently-discovered transition-metal pentatellurides can reach the ultra-quantum limit in low magnetic fields and serve as good candidates for achieving such a combination. Here, we report evidences of density wave and metal-insulator transition in HfTe5 induced by intense magnetic fields. Using the nonlinear transport technique, we detect a distinct nonlinear conduction behavior in the longitudinal resistivity within the a-c plane, corresponding to the formation of a density wave induced by magnetic fields. In high fields, the onset of the nonlinear conduction in the Hall resistivity indicates an impurity-pinned magnetic freeze-out as the possible origin of the insulating behavior. These frozen electrons can be gradually re-activated into mobile states above a threshold electric field. These experimental evidences call for further investigations into the underlying mechanism for the bulk quantum Hall effect and field-induced phase transtions in pentatellurides.",2311.11517v1 2023-11-29,Lateral NbS$_2$/MoS$_2$/NbS$_2$ transistors: physical modeling and performance assessment,"Reducing the contact resistance of field-effect transistors based on two-dimensional materials is one of the key improvements required to to enable the integration of such transistors in an industrially relevant process. Suitably designed lateral heterojunctions provide an opportunity to independently tailor the contact and channel properties and to mitigate the problem of high contact resistance. Inspired by the recent experimental demonstration of a two-dimensional $p$-type Schottky barrier, here we use quantum transport simulations to estimate the performance of $p$-type transistors in which the channel consists of a lateral heterostructure of NbS$_2$/MoS$_2$/NbS$_2$ (semimetal-semiconductor-semimetal). We find that the gate alignment with the channel is a critical design parameter, strongly influencing the capability of the gate to modulate the Schottky barrier at the MoS$_2$/NbS$_2$ interfaces. This effect is also found to significantly affect the scaling behavior of the device.",2311.18031v1 2024-02-23,Electrical Scanning Probe Microscope Measurements Reveal Surprisingly High Dark Conductivity in Y6 and PM6:Y6 and Non-Langevin Recombination in PM6:Y6,"We used broadband local dielectric spectroscopy (BLDS), an electric force microscopy technique, to make non-contact measurements of conductivity in the dark and under illumination of PM6:Y6 and Y6 prepared on ITO and PEDOT:PSS/ITO. Over a range of illumination intensities, BLDS spectra were acquired and fit to an impedance model of the tip-sample interaction to obtain a sample resistance and capacitance. By comparing two descriptions of cantilever friction, an impedance model and a microscopic model, we connected the sample resistance inferred from impedance modeling to a microscopic sample conductivity. A charge recombination rate was estimated from plots of the conductivity versus light intensity and found to be sub-Langevin. The dark conductivity was orders of magnitude higher than expected from Fermi-level equilibration of the PM6:Y6 with the substrate, suggesting that dark carriers may be a source of open-circuit voltage loss in PM6:Y6.",2402.15501v1 2021-05-07,Integrating van der Waals materials on paper substrates for electrical and optical applications,"Paper holds the promise to replace silicon substrates in applications like internet of things or disposable electronics that require ultra-low-cost electronic components and an environmentally friendly electronic waste management. In the last years, spurred by the abovementioned properties of paper as a substrate and the exceptional electronic, mechanical and optical properties of van der Waals (vdW) materials, many research groups have worked towards the integration of vdW materials-based devices on paper. Recently, a method to deposit a continuous film of densely packed interconnects of vdW materials on paper by simply rubbing the vdW crystals against the rough surface of paper has been presented. This method utilizes the weak interlayer vdW interactions and allows cleaving of the crystals into micro platelets through the abrasion against the paper. Here, we aim to illustrate the general character and the potential of this technique by fabricating films of 39 different vdW materials (including superconductors, semi-metals, semiconductors, and insulators) on standard copier paper. We have thoroughly characterized their optical properties showing their high optical quality: one can easily resolve the absorption band edge of semiconducting vdW materials and even the excitonic features present in some vdW materials with high exciton binding energy. We also measured the electrical resistivity for several vdW materials films on paper finding exceptionally low values, which are in some cases, orders of magnitude lower than those reported for analogous films produced by inkjet printing. We finally demonstrate the fabrication of field-effect devices with vdW materials on paper using the paper substrate as an ionic gate.",2105.03486v1 2017-06-29,Origin of Contact Resistance at Ferromagnetic Metal-Graphene Interfaces,"Edge contact geometries are thought to yield ultralow contact resistances in most non-ferromagnetic metal-graphene interfaces owing to their large metal-graphene coupling strengths. Here, we examine the contact resistance of edge- versus surface-contacted ferromagnetic metal-graphene interfaces (i.e. nickel- and cobalt-graphene interfaces) using both single-layer and few-layer graphene. Good qualitative agreement is obtained between theory and experiment. In particular, in both theory and experiment, we observe that the contact resistance of edge-contacted ferromagnetic metal-graphene interfaces is much lower than that of surface-contacted ones, for all devices studied and especially for the single-layer graphene systems. We show that this difference in resistance is not due to differences in the metal-graphene coupling strength, which we quantify using Hamiltonian matrix elements. Instead, the larger contact resistance in surface contacts results from spin filtering at the interface, in contrast to the edge-contacted case where both spins are transmitted. Temperature-dependent resistance measurements beyond the Curie temperature TC show that the spin degree of freedom is indeed important for the experimentally measured contact resistance. These results show that it is possible to induce a large change in contact resistance by changing the temperature in the vicinity of TC, thus paving the way for temperature-controlled switches based on spin.",1706.09591v1 2023-09-22,Non-equilibrium Thermal Resistance of Interfaces Between III-V Compounds,"Interfacial thermal resistance has been often estimated and understood using the Landauer formalism that assumes incident phonons with equilibrium distribution. However, previous studies suggest that phonons are out-of-equilibrium near the interface because of the heat flow through the leads and the scattering of phonons by the interface. In this paper, we report a systematic study on how vibrational spectra mismatch affects the degree of phonon non-equilibrium near an interface, how fast it is relaxed as the phonons diffuse into a lead, and the overall interfacial thermal resistance from the non-equilibrium phonons. Our discussion is based on the solution of the Peierls-Boltzmann transport equation with ab initio inputs for 36 interfaces between semi-infinite group-III (Al, Ga, In) and group-V (P, As, Sb) compound semiconductor leads. The simulation reveals that the non-equilibrium phonons cause significant interfacial thermal resistance for all 36 interfaces, making the overall interfacial thermal resistance two to three times larger than that predicted by the Landauer formalism. We observe a clear trend that the degree of phonon non-equilibrium near an interface and the interfacial thermal resistance from the non-equilibrium phonons increase as the mismatch of the Debye temperature of two lead materials increases. This contrasts with Landauer formalism's predictions, which show no correlation with the Debye temperature mismatch. The relaxation length of the phonon non-equilibrium varies significantly from 50nm to 1.5um depending on the combination of the lead materials. The relaxation length is proportional to the phonon mean free path of the corresponding lead material but also largely depends on the material in the opposite lead. This suggests the relaxation length cannot be considered an intrinsic property of the corresponding lead material.",2309.13187v1 2003-10-28,On magnetic field generation in Kolmogorov turbulence,"We analyze the initial, kinematic stage of magnetic field evolution in an isotropic and homogeneous turbulent conducting fluid with a rough velocity field, v(l) ~ l^alpha, alpha<1. We propose that in the limit of small magnetic Prandtl number, i.e. when ohmic resistivity is much larger than viscosity, the smaller the roughness exponent, alpha, the larger the magnetic Reynolds number that is needed to excite magnetic fluctuations. This implies that numerical or experimental investigations of magnetohydrodynamic turbulence with small Prandtl numbers need to achieve extremely high resolution in order to describe magnetic phenomena adequately.",0310780v2 1999-08-04,Polarization fields in nitride nanostructures: ten points to think about,"Macroscopic polarization, both of intrinsic and piezoelectric nature, is unusually strong in III-V nitrides, and the built in electric fields in the layers of nitride-based nanostructures, stemming from polarization changes at heterointerfaces, have a major impact on the properties of single and multiple quantum wells, high mobility transistors, and thin films. The concepts involved in the theory and applications of polarization in nitrides have encountered some resistance in the field. Here we discuss critically ten ``propositions'' aimed at clarifying the main controversial issues.",9908060v1 2001-02-06,"Observation of superconductivity in Y$_2$PdGe$_3$, structurally same as MgB$_2$","The results of electrical resistance (1.4 - 300 K), magnetization (2-300 K) and heat-capacity (2 - 50 K) measurements in Y$_2$PdGe$_3$, found to crystallize in a AlB$_2$-derived hexagonalstructure, are reported. The results establish that this compound is superconducting below 3 K. This obervation is interesting considering that this compound is the first superconductor among the ternary members derived from the hexagonal AlB$_2$ structure. With superconductivity being uncommon even among binary alloys derived from AlB$_2$ structure and with recent excitement on the observation of high temperature superconductivity in Mg$B_2$, this finding gains importance.",0102110v1 2002-05-08,Complex Quantum Phenomena in a Bilayered Calcium Ruthenate,"Ca$_3$Ru$_2$O$_7$ undergoes an antiferromagnetic transition at $T_{\text{N}}=56 $K, followed by a Mott-like (MI) transition at $T_{\text{MI}}=48$ K. This nonmetallic ground state, with a charge gap of 0.1 eV, is suppressed by a highly anisotropic metamagnetic transition that leads to a fully spin-polarized metallic state. We report the observation of Shubnikov-de Haas oscillations in the \textit{gapped} state, colossal magnetoresistance in the inter-plane resistivity with a large anisotropy different from that observed in the magnetization, and non-Fermi liquid behavior in the metallic state at high magnetic fields.",0205151v1 2002-06-10,Realization of La2MnVO6: Search for half-metallic antiferromagnetism?,"Single-phase polycrystalline La2MnVO6 samples were synthesized by arc melting and characterized by X-ray diffraction, magnetization and resistivity measurements. We find that the compound has cubic (space group), partly ordered double perovskite structure. The sample exhibits ferrimagnetic behavior and variable-range hopping conductivity. We conclude based on the magnetic properties that both Mn and V ions are trivalent; moreover, the Mn3+ ions are in a high-spin state, which is the reason that the compound is not a half-metallic antiferromagnet.",0206146v1 2002-07-09,Perspectives of superconducting MgB2 for microwave applications,"We discuss the temperature, frequency, and power-dependent surface resistance of the boride superconductor MgB2 in relation to possible applications for passive microwave devices. The data available in the literature are compared with results for polycrystalline Nb3Sn and epitaxial YBa2Cu3O7-x, which are representative of the classical and cuprate superconductors. MgB2 displays all specific features that make superconductors attractive for high-performance devices, even though the fabrication technology is not yet mature. We attempt to identify promising areas of applications, as well as material requirements, which could further promote the attractiveness of the new superconductor in this field.",0207226v1 2002-08-15,Superconductivity in Ba_2Sn_3Sb_6 and SrSn_3Sb_4,"Resistivity and ac magnetic susceptibility measurements on Ba2Sn3Sb6 and SrSn3Sb4 indicate that these Zintl compounds display a transition to a superconducting phase at Tc = 3.9 K. The Meissner effect was observed for Ba2Sn3Sb6 under an applied field of 25 Oe. The signatures for superconductivity, such as high and low velocity conduction electrons and lone pairs, are present for both of these compounds.",0208313v1 2002-11-22,Correlations and Semimetallic Behaviors in Pyrochlore Oxide Cd2Re2O7,"Electronic properties of the metallic pyrochlore oxide Cd2Re2O7 are studied by means of electrical resistivity and Hall measurements. Semimetallic band structures are revealed as expected from band structure calculations. It is found that large changes in carrier density and mass occur at the structural phase transition at Ts1 = 200 K. A large mass enhancement is observed, particularly for the high-temperature phase with the ideal pyrochlore structure, suggesting that an anomalous correlation has an important effect on the itinerant electrons in the pyrochlore lattice.",0211517v1 2004-02-02,Dielectric responses of the layered cobalt oxysulfide Sr_2Cu_2CoO_2S_2 with CoO_2 square-planes,"We have studied the dielectric responses of the layered cobalt oxysulfide Sr$_2$Cu$_2$CoO$_2$S$_2$ with the CoO$_2$ square-planes. With decreasing temperature below the N\'eel temperature, the resistivity increases like a semiconductor, and the thermopower decreases like a metal. The dielectric constant is highly dependent on temperature, and the dielectric relaxation is systematically changed with temperature, which is strongly correlated to the magnetic states. These behaviors suggest that carriers distributed homogeneously in the paramagnetic state at high temperatures are expelled from the antiferromagnetically ordered spin domain below the N\'eel temperature.",0402034v1 2005-01-28,Ce doping in T-La2CuO4 films: Broken electron-hole symmetry for high-Tc superconductivity,"We attempted Ce doping in La2CuO4 with the K2NiF4 (T) structure by molecular beam epitaxy. At low growth temperature and with an appropriate substrate choice, we found that Ce can be incorporated into the K2NiF4 lattice up to x ~ 0.06, which had not yet been realized in bulk synthesis. The doping of Ce makes T-La2-xCexCuO4 more insulating, which is in sharp contrast to Ce doping in La2CuO4 with the Nd2CuO4 structure, which makes the compounds superconducting. The observed smooth increase in resistivity from hole-doped side (T-La2-xSrxCuO4) to electron-doped side (T-La2-xCexCuO4) indicates that electron-hole symmetry is broken in the T-phase materials.",0501703v1 2005-09-05,"Large magnetoresistance and magnetocaloric effect above 70 K in Gd2Co2Al, Gd2Co2Ga and Gd7Rh3","The electrical resistivity, magnetization and heat-capacity behavior of the Gd-based compounds, Gd2Co2Al, Gd2Co2Ga and Gd7Rh3, ordering magnetically at TC= 78 K, TC= 76 K and TN= 140 K have been investigated as a function of temperature and magnetic field. All these compounds are found to show large magnetoresistance (with a negative sign) in the paramagnetic state at rather high temperatures with the magnitude peaking at respective magnetic ordering temperatures. There is a corresponding behavior in the magnetocaloric effect as inferred from the entropy derived from these data.",0509107v1 2006-10-11,"Intergrain connectivity and resistive broadening in vortex state: a comparison between MgB2, NbSe2 and Bi2Sr2Ca2Cu3O10 superconductors","Magnetoresistance and radio frequency penetration depth techniques are used to study grain connectivity and broadening of superconducting transition. We study and compare these issues in clean polycrytalline samples of three different superconducting systems e.g. MgB2, NbSe2 and Bi2Sr2Ca2Cu3O10. From the rf response, the bulk pinning force constant is evaluated. From high field transport measurements, H-T phase diagram is ascertained for the three systems with varying degrees of fluctuation and connectivity.",0610295v1 2007-03-25,Novel dynamical effects and glassy response in strongly correlated electronic system,"We find an unconventional nucleation of low temperature paramagnetic metal (PMM) phase with monoclinic structure from the matrix of high-temperature antiferromagnetic insulator (AFI) phase with tetragonal structure in strongly correlated electronic system $BaCo_{0.9}Ni_{0.1}S_{1.97}$. Such unconventional nucleation leads to a decease in resistivity by several orders with relaxation at a fixed temperature without external perturbation. The novel dynamical process could arise from the competition of strain fields, Coulomb interactions, magnetic correlations and disorders. Such competition may frustrate the nucleation, giving rise to a slow, nonexponential relaxation and ""physical aging"" behavior.",0703647v1 2007-07-05,Anomalous exchange coupling in transition-metal-oxide based superlattices with antiferromagnetic spacer layers,"A direct correlation is seen between the coercive field (HC) and the magnetic-field-dependent resistivity (MR) in SrMnO3/SrRuO3 superlattices of perpendicular magnetic anisotropy. The magnetoresistance shows a sharp jump at Hc for in-plane current and the out-of-plane magnetic field. Both HC and high-field MR also oscillate with the thickness of the SrMnO3 spacer layers separating the metallic ruthenate. Since the spacer in these superlattices has no mobile carriers to facilitate an oscillatory coupling, we attribute the observed behavior to the spin-polarized quantum tunneling of electrons between the ferromagnetic layers and antiferromagnetically ordered t2g spins of SrMnO3.",0707.0768v1 2007-08-10,Coherent quasiparticle transport in grain boundary junctions employing high-Tc superconductors,"Magneto-fluctuations of the normal resistance RN have been reproducibly observed in YBa2Cu3O7-d biepitaxial grain boundary junctions at low temperatures. We attribute them to mesoscopic transport in narrow channels across the grain boundary line, occurring in an unusual energy regime. The Thouless energy appears to be the relevant energy scale. Possible implications on the understanding of coherent transport of quasiparticles in HTS and of the dissipation mechanisms are discussed.",0708.1448v1 2007-09-26,Single crystal growth and anisotropy of CeRuPO,"We report on the single crystal growth of the ferromagnetic Kondo lattice system CeRuPO using a Sn flux method. Magnetic susceptibility and electrical resistivity measurements indicate strong anisotropy of this structurally layered compound. They evidence that the magnetic moments order ferromagnetically along the c-direction of the tetragonal unit cell, whereas the crystal electric field (CEF) anisotropy favors the ab-plane. Therefore, CeRuPO presents the unusual case within rare earth systems, where the anisotropy of the interionic exchange interaction overcomes the single ion anisotropy due to the CEF interaction.",0709.4144v2 2007-11-30,Large voltage from spin pumping in magnetic tunnel junctions,"We studied the response of a ferromagnet-insulator-normal metal tunnel structure under an external oscillating radio frequency (R.F.) magnetic field. The D. C. voltage across the junction is calculated and is found not to decrease despite the high resistance of the junction; instead, it is of the order of $\mu V$ to $100\mu V$, much larger than the experimentally observed value (100 nano-V) in the ""strong coupled"" ohmic ferromagnet-normal metal bilayers. This is consistent with recent experimental results in tunnel structures, where the voltage is larger than $\mu V$s. The damping and loss of an external RF field in this structure is calculated.",0711.4939v1 2008-01-07,High Performance Thermal Interface Technology Overview,"An overview on recent developments in thermal interfaces is given with a focus on a novel thermal interface technology that allows the formation of 2-3 times thinner bondlines with strongly improved thermal properties at lower assembly pressures. This is achieved using nested hierarchical surface channels to control the particle stacking with highly particle-filled materials. Reliability testing with thermal cycling has also demonstrated a decrease in thermal resistance after extended times with longer overall lifetime compared to a flat interface.",0801.1046v1 2008-01-17,Stability of RVB hole stripes in high-temperature superconductors,"Indications of density-wave states in underdoped cuprates, coming from recent STM (scanning tunneling microscopy) and Hall-resistance measurements, have raised new concerns whether stripes could be stabilized in the superconducting phase of cuprate materials, even in the absence of antiferromagnetism. Here, we investigate this issue using state-of-the-art quantum Monte Carlo calculations of a $t-J$ model. In particular we consider the stability of unidirectional hole domains in a modulated superconducting background, by taking into account the effect of tetragonal-lattice distortions, next-nearest neighbor hopping and long-range Coulomb repulsion.",0801.2722v2 2008-08-03,Superconductivity in Yttrium Iron Oxyarsenide System,"Iron-based oxypnictides substituted with yttrium have been prepared via a conventional solid state reaction. The product after first 50 hours of reaction showed diamagnetic-like transition at around 10 K but was not superconducting, while additional 72 hours of high temperature heat treatment was required to yield superconducting sample which was doped with fluoride. Temperature dependence of the susceptibility shows both screening and Meissner effect at around 10 K, while resistance as a function of temperature displayed a drop at around the same temperature.",0808.0288v2 2008-09-16,"Interface heat transfer between crossing carbon nanotubes, and the thermal conductivity of nanotube pellets","We theoretically compute the interface thermal resistance between crossing single walled carbon nanotubes of various chiralities, using an atomistic Green's function approach with semi-empirical potentials. The results are then used to model the thermal conductivity of three dimensional nanotube pellets in vacuum. For an average nanotube length of 1 $\mu$m, the model yields an upper bound for the thermal conductivity of densely compacted pellets, of the order of a few W/m-K. This is in striking contrast with the ultra-high thermal conductivity reported on individually suspended nanotubes. The results suggest that nanotube pellets might have an application as thermal insulators.",0809.2660v1 2008-10-29,High-Mobility Few-Layer Graphene Field Effect Transistors Fabricated on Epitaxial Ferroelectric Gate Oxides (Supplementary Information),"Supplementary Information to arXiv:0810.4466: 1. Characterizations of Pb(Zr_0.2Ti_0.8)O_3 (PZT) films. 2. Substrate preparation before the exfoliation of graphene. 3. The band structure of FLG. 4. Dielectric constant measurements of PZT. 5. rho(V_g) and R_H(V_g) fitting inside the band overlap regime. 6. The deformation potential of longitudinal acoustic (LA) phonons in graphene. 7. Resistivity and Hall measurements of a SiO_2-gated FLG.",0810.5339v1 2008-12-20,Mobility Extraction and Quantum Capacitance Impact in High Performance Graphene Field-effect Transistor Devices,"The field-effect mobility of graphene devices is discussed. We argue that the graphene ballistic mean free path can only be extracted by taking into account both, the electrical characteristics and the channel length dependent mobility. In doing so we find a ballistic mean free path of 300nm at room-temperature for a carrier concentration of ~1e12/cm2 and that a substantial series resistance of around 300ohmum has to be taken into account. Furthermore, we demonstrate first quantum capacitance measurements on single-layer graphene devices.",0812.3927v1 2009-01-07,Electrically Controlled Magnetic Memory and Programmable Logic based on Graphene/Ferromagnet Hybrid Structures,"It has been shown that the combining of the electrical effect on the exchange bias field with giant magneto-resistance effect of the graphene/ferromagnet hybrid structures reveals a new non-volatile magnetic random access memory device conception. In such device an electric bias realizes the writing bits instead a magnetic field of remote word line with high energy consumption. Interplay of two graphene mediated exchange bias fields applied to different sides of free ferromagnet results in programable logic operations that depends on specific realization of the structure.",0901.0926v1 2009-03-21,Graphite in the bi-layer regime: in-plane transport,"An interplay between the increase in the number of carriers and the decrease in the scattering time is expected to result in a saturation of the in-plane resistivity, $\rho_{ab}$, in graphite above room temperature. Contrary to this expectation, we observe a pronounced increase in $\rho_{ab}$ in the interval between 300 and 900 K. We provide a theory of this effect based on intervalley scattering of charge carriers by high-frequency, graphene-like optical phonons.",0903.3646v2 2009-04-22,Emergence of dissipative structures in current-carrying superconducting wires,"We discuss the emergence of a spontaneous temperature and critical current spatial modulation in current-carrying high temperature superconducting wire. The modulation of the critical current along the wire on a scale of 3 - 10 mm forces a fraction of the transport current to crisscross the resistive interface between the superconducting film and normal metal stabilizer attached to it. This generates additional heat that allows such a structure to be self sustainable. Stability and the conditions for experimental observation of this phenomenon are also discussed.",0904.3474v1 2009-04-23,"Crystal growth, structure and ferromagnetic properties of a Ce3Pt23Si11 single crystal","A high-quality single crystal of Ce3Pt23Si11 has been grown using the Czochralski method. The crystal structure is presented and the chemical composition has been checked using an electron microprobe analyzer. Measurements of the electrical resistivity and magnetic susceptibility performed at low temperature show a ferromagnetic transition at Tc = 0.44 K.",0904.3720v1 2009-05-29,Growth of Sr1-xCaxRuO3 thin films by metalorganic aerosol deposition,"We report the growth of thin films of Sr1-xCaxRuO3 on SrTiO3 and MgO substrates by metalorganic aerosol deposition. The structure and microstructure is characterized by X-ray diffraction and room-temperature scanning tunnelling microscopy (STM), respectively. STM indicates in-plane epitaxy and a small surface roughness for films on SrTiO3. The high-quality of the films is supported by large residual resistivity ratios up to 29.",0905.4896v2 2009-09-07,Anomalous magnetotransport and cyclotron resonance of high mobility magnetic 2DHGs in the quantum Hall regime,"Low temperature magnetotransport measurements and far infrared transmission spectroscopy are reported in molecular beam epitaxial grown two-dimensional hole systems confined in strained InAs quantum wells with magnetic impurities in the channel. The interactions of the free holes spin with the magnetic moment of 5/2 provided by manganese features intriguing localization phenomena and anomalies in the Hall and the quantum Hall resistance. In magnetic field dependent far infrared spectroscopy measurements well pronounced cyclotron resonance and an additional resonance are found that indicates an anticrossing with the cyclotron resonance.",0909.1124v1 2010-08-15,Unconventional Anomalous Hall Effect in the Metallic Triangular-Lattice Magnet PdCrO2,"We experimentally reveal an unconventional anomalous Hall effect (UAHE) in a quasi-two-dimensional triangular-lattice antiferromagnet PdCrO2. Using high quality single crystals of PdCrO2, we found that the Hall resistivity deviates from the conventional behavior below T* = 20 K, noticeably lower than TN = 37.5 K, at which Cr^{3+} (S=3/2) spins order in a 120 degree structure. In view of the theoretical expectation that the spin chirality cancels out in the simplest 120 degree spin structure, we discuss required conditions for the emergence of UAHE within Berry-phase mechanisms.",1008.2503v1 2010-08-27,Metal-nonmetal transition in LixCoO2 thin film and thermopower enhancement at high Li concentration,"We investigate the transport properties of LixCoO2 thin films whose resistivities are nearly an order of magnitude lower than those of the bulk polycrystals. A metal-nonmetal transition occurs at ~0.8 in a biphasic domain, and the Seebeck coefficient (S) is drastically increased at ~140 K (= T*) with increasing the Li concentration to show a peak of magnitude ~120 \muV/K in the S-T curve of x = 0.87. We show that T* corresponds to a crossover temperature in the conduction, most likely reflecting the correlation-induced temperature dependence in the low-energy excitations.",1008.4635v1 2010-10-21,Atomistic quantum transport modeling of metal-graphene nanoribbon heterojunctions,"We calculate quantum transport for metal-graphene nanoribbon heterojunctions within the atomistic self-consistent Schr\""odinger/Poisson scheme. Attention is paid on both the chemical aspects of the interface bonding as well the one-dimensional electrostatics along the ribbon length. Band-bending and doping effects strongly influence the transport properties, giving rise to conductance asymmetries and a selective suppression of the subband formation. Junction electrostatics and p-type characteristics drive the conduction mechanism in the case of high work function Au, Pd and Pt electrodes, while contact resistance becomes dominant in the case of Al.",1010.4393v1 2010-11-02,Spin connection and boundary states in a topological insulator,"We study the surface resistivity of a three-dimensional topological insulator when the boundaries exhibit a non trivial curvature. We obtain an analytical solution for a spherical topological insulator, and we show that a non trivial quantum spin connection emerges from the three dimensional band structure. We analyze the effect of the spin connection on the scattering by a bump on a flat surface. Quantum effects induced by the geometry lead to resonances when the electron wavelength is comparable to the size of the bump.",1011.0565v1 2010-11-20,Imaging Dissipation and Hot Spots in Carbon Nanotube Network Transistors,"We use infrared thermometry of carbon nanotube network (CNN) transistors and find the formation of distinct hot spots during operation. However, the average CNN temperature at breakdown is significantly lower than expected from the breakdown of individual nanotubes, suggesting extremely high regions of power dissipation at the nanotube junctions. Statistical analysis and comparison with a thermal model allow the extraction of the average tube-tube junction thermal resistance, ~4.4x10^11 K/W (thermal conductance ~2.27 pW/K). This indicates that nanotube junctions have a much greater impact on CNN transport, dissipation, and reliability than extrinsic factors such as low substrate thermal conductivity.",1011.4551v2 2011-05-16,Coulomb drag in graphene,"We calculate theoretically the Coulomb drag resistivity for two graphene monolayers spatially separated by a distance ""$d$"". We show that the frictional drag induced by inter-layer electron-electron interaction goes asymptotically as $T^2/n^3$ and $T^2 \ln(n)/n$ in the high-density ($k_F d \gg 1$) and low-density ($k_F d \ll 1$) limits, respectively.",1105.3203v2 2011-07-23,Modified exponential I(U) dependence and optical efficiency of AlGaAs SCH lasers in computer modeling with Synopsys TCAD,"Optical and electrical characteristics of AlGaAs lasers with separate confinement heterostructures are modeled by using Synopsys's Sentaurus TCAD, and open source software. We propose a modified exponential $I-V$ dependence to describe electrical properties. A simple analytical, phenomenological model is found to describe optical efficiency, $\eta$, with a high accuracy, by using two parameters only. A link is shown between differential electrical resistivity $r=dU/dI$ just above the lasing offset voltage, and the functional $\eta(U)$ dependence.",1107.4668v1 2011-08-20,Demonstration of Forward Inter-band Tunneling in GaN by Polarization Engineering,"We report on the design, fabrication, and characterization of GaN interband tunnel junction showing forward tunneling characteristics. We have achieved very high forward tunneling currents (153 mA/cm2 at 10 mV, and 17.7 A/cm2 peak current) in polarization-engineered GaN/InGaN/GaN heterojunction diodes grown by plasma assisted molecular beam epitaxy. We also report the observation of repeatable negative differential resistance in interband III-Nitride tunnel junctions, with peak-valley current ratio (PVCR) of 4 at room temperature. The forward current density achieved in this work meets the typical current drive requirements of a multi-junction solar cell.",1108.4075v1 2012-04-10,Tunneling conduction in graphene/(poly)vinyl alcohol composites,"Graphene/(Poly)vinyl alcohol (PVA) composite film with thickness $60 \mu m$ were synthesized by solidification of a PVA solution comprising of dispersed graphene nanosheets. The close proximity of the graphene sheets enables the fluctuation induced tunneling of electrons to occur from one sheet to another. The dielectric data show that the present system can be simulated to a parallel resistance-capacitor network. The high frequency exponent of the frequency variation of the ac conductivity indicates that the charge carriers move in a two-dimensional space. The sample preparation technique will be helpful for synthesizing flexible conductors.",1204.2126v2 2012-07-27,Theoretical model of structure-dependent conductance crossover in disordered carbon,"We analyze the effects of sp^2/sp^3 bond-aspect ratio on the transport properties of amorphous carbon quasi-1D structures where structural disorder varies in a very non-linear manner with the effective bandgap. Using a tight-binding approach the calculated electron transmission showed a high probability over a wide region around the Fermi-level for sp^2-rich carbon and also distinct peaks close to the band edges for sp^3-rich carbon structures. This model shows a sharp rise of the structure resistance with the increase of sp^3C % followed by saturation in the wide bandgap regime for carbon superlattice-like structures and suggests the tuneable characteristic time of carbon-based devices.",1207.6478v1 2012-11-22,Physical properties and band structure of reactive molecular beam epitaxy grown oxygen engineered HfO$_{2\pm x}$,"We have conducted a detailed thin film growth structure of oxygen engineered monoclinic HfO$_{2\pm x}$ grown by reactive molecular beam epitaxy (MBE). The oxidation conditions induce a switching between ($\bar{1}11$) and (002) texture of hafnium oxide. The band gap of oxygen deficient hafnia decreases with increasing amount of oxygen vacancies by more than 1 eV. For high oxygen vacancy concentrations, defect bands form inside the band gap that induce optical transitions and $p$-type conductivity. The resistivity changes by several orders of magnitude as a function of oxidation conditions. Oxygen vacancies do not give rise to ferromagnetic behavior.",1211.5215v1 2013-05-21,High sensitive quasi freestanding epitaxial graphene gassensor on 6H-SiC,"We have measured the electrical response to NO$_2$, N$_2$, NH$_3$ and CO for epitaxial graphene and quasi freestanding epitaxial graphene on 6H-SiC substrates. Quasi freestanding epitaxial graphene shows a 6 fold increase in NO2 sensitivity compared to epitaxial graphene. Both samples show a sensitivity better than the experimentally limited 1 ppb. The strong increase in sensitivity of quasi freestanding epitaxial graphene can be explained by a Fermi-energy close to the Dirac Point leading to a strongly surface doping dependent sample resistance. Both sensors show a negligible sensitivity to N$_2$, NH$_3$ and CO.",1305.4737v1 2013-09-04,Enhancing high-temperature thermoelectric properties of PtAs2 by Rh doping,"The effects of Rh doping on the thermoelectric properties of Pt1-xRhxAs2 (x = 0, 0.005, and 0.01) with pyrite structure were studied by conducting measurements of electrical resistivity rho, Seebeck coefficient S, and thermal conductivity kappa. The sample with x = 0.005 exhibited large S and low rho, resulting in a maximum power factor (S^2/rho) of 65 muW/cmK^2 at 440 K. The peculiarly shaped ""corrugated flat band"" predicted for PtSb2 might explain the enhanced thermoelectric properties of doped PtAs2.",1309.0939v1 2013-10-06,Charge transport through graphene junctions with wetting metal leads,"Graphene is believed to be an excellent candidate material for next-generation electronic devices. However, one needs to take into account the nontrivial effect of metal contacts in order to precisely control the charge injection and extraction processes. We have performed transport calculations for graphene junctions with wetting metal leads (metal leads that bind covalently to graphene) using nonequilibrium Green's functions and density functional theory. Quantitative information is provided on the increased resistance with respect to ideal contacts and on the statistics of current fluctuations. We find that charge transport through the studied two-terminal graphene junction with Ti contacts is pseudo-diffusive up to surprisingly high energies.",1310.1640v1 2013-11-17,Giant magnetothermopower in charge ordered Nd0.75Na0.25MnO3,"We report magnetization, resistivity and thermopower in the charge-orbital ordered antiferromagnet Nd0.75Na0.25MnO3. Magnetic-field induced collapse of antiferromagnetism is found to be accompanied by a giant negative magnetothermopower (= 80-100% for a field change of 5T) over a wide temperature (T = 60-225K) and giant magnetoresistance. While the field-induced metamagnetic transition in magnetization is reversible upon field-cycling at T > 40 K, it is irreversible at lower temperatures and this has impact on magnetoresistance, magnetothermopower as well as change in the temperature of the sample. Our results indicate high sensitivity of thermopower to changes in the magnetic state of the sample.",1311.4165v1 2014-02-05,Selective molecular capture mechanism in carbon nanotube networks,"Recent air pollution issues have raised significant attention to develop efficient air filters, and one of the most promising candidates is that enabled by nanofibers. We explore here selective molecular capture mechanism for volatile organic compounds in carbon nanotube networks by performing atomistic simulations. The results are discussed with respect to the two key parameters that define the performance of nanofiltration, i.e. the capture efficiency and flow resistance, which validate the advantage of carbon nanotube networks with high surface-to-volume ratio and atomistically smooth surfaces. We also reveal the important roles of interfacial adhesion and diffusion that govern selective gas transport through the network.",1402.1011v1 2016-01-06,Effect of SW defect on structural and transport properties of silicene nanoribbons,"Using density functional theory and non-equilibrium Greens function technique, we performed theoretical investigations on the structural and transport properties of zigzag silicene nanoribbons with Stone-Wales defect. The calculated formation energy is significantly lower than that of graphene and silicene, which implies the high stability of such defect in SiNRs. Negative differential resistance can be observed within certain bias voltage range in both perfect and SW defected SiNRs. In order to elucidate the mechanism the NDR behavior,the transmission spectra and molecular projected self-consistent Hamiltonian states are discussed in details.",1601.01053v1 2016-01-30,Slippery but tough - the rapid fracture of lubricated frictional interfaces,"We study the onset of friction for rough contacting blocks whose interface is coated with a thin lubrication layer. High speed measurements of the real contact area and stress fields near the interface reveal that propagating shear cracks mediate lubricated frictional motion. While lubricants reduce interface resistances, surprisingly, they significantly increase energy dissipated, $\Gamma$, during rupture. Moreover, lubricant viscosity affects the onset of friction but has no effect on $\Gamma$. Fracture mechanics provide a new way to view the otherwise hidden complex dynamics of the lubrication layer.",1602.00085v2 2016-10-09,Physical properties of KMgBi single crystals,"KMgBi single crystals are grown by using the Bi flux successfully. KMgBi shows semiconducting behavior with a metal-semiconductor transition at high temperature region and a resistivity plateau at low temperature region, suggesting KMgBi could be a topological insulator with a very small band gap. Moreover, KMgBi exhibits multiband feature with strong temperature dependence of carrier concentrations and mobilities.",1610.02699v2 2017-06-27,Influence of Heat Treatment on the Corrosion Behavior of Purified Magnesium and AZ31 Alloy,"Magnesium and its alloys are ideal for biodegradable implants due to their biocompatibility and their low-stress shielding. However, they can corrode too rapidly in the biological environment. The objective of this research was to develop heat treatments to slow the corrosion of high purified magnesium and AZ31 alloy in simulated body fluid at 37{\deg}C. Heat treatments were performed at different temperatures and times. Hydrogen evolution, weight loss, PDP, and EIS methods were used to measure the corrosion rates. Results show that heat treating can increase the corrosion resistance of HP-Mg by 2x and AZ31 by 10x.",1706.08663v1 2017-12-06,Superconductivity in the ternary compound SrPt$_{10}$P$_4$ with complex new structure,"We report superconductivity at 1.4K in the ternary SrPt$_{10}$P$_4$ with a complex new structure. SrPt$_{10}$P$_4$ crystallizes in a monoclinic space-group C2/c (\#15) with lattice parameters a= 22.9151(9)$\AA$, b= 13.1664(5)$\AA$, c=13.4131(5)$\AA$, and $\beta$= 90.0270(5)${^\circ}$. Bulk superconductivity in the samples has been demonstrated through resistivity, ac susceptibility, and heat capacity measurements. High pressure measurements have shown that the superconducting T$_C$ is systematically suppressed upon application of pressure, with a dT$_C$/dP coefficient of -0.016 K/GPa.",1712.02010v1 2018-03-06,Comparative study on magnetoresistance of carbon-cobalt nanocomposite thin films grown by pulsed laser deposition,"We present a comparative study on the influence of applied magnetic field on the resistance of $C_{1-x}Co_x$ thin films (with $x=0.1$, $0.15$ and $0.2$) grown on $Si$ substrate by pulsed laser deposition technique. It is found that the behavior of magnetoresistance (MR) drastically depends on the temperature. Namely, at low temperatures MR is positive and its behavior is governed by the field mediated weak localization scenario. While at high temperatures MR turns negative and its behavior is dominated by electron scattering on ferromagnetic cobalt atoms.",1803.02064v1 2018-04-27,Emergent antiferromagnetism of YTiO3 in YTiO3-CaTiO3 superlattices,"Transport and magnetoresistance measurements are performed on metallic, high-carrier density YTiO3-CaTiO3 superlattices as a probe towards the investigation of an emergent magnetic order of YTiO3. On varying the thickness of YTiO3 while keeping the CaTiO3 layer thickness constant in the superlattices, a low-temperature upturn in sheet-resistance, a non-Fermi liquid-like charge transport and positive magnetoresistance are observed. Analyses of the origin of such effects suggest that a unique antiferromagnetic order is realized in the ultra-thin, epitaxially strained YTiO3 layers, which corroborates well with some recent theoretical predictions in this regard.",1804.10333v1 2018-10-01,Poly(ionic liquid)-Derived Carbon with Site-Specific N-Doping and Biphasic Heterojunction for Enhanced CO2 Capture and Sensing,"CO2 capture is a pressing global environmental issue that drives scientists to develop creative strategies for tackling this challenge. The concept in this contribution is to produce site specific nitrogen doping in microporous carbon fibers. It creates a carbon/carbon heterojunction by using poly(ionic liquid) (PIL) as soft activation agent that deposits nitrogen species exclusively on the skin of commercial microporous carbon fibers. Such carbon-based biphasic heterojunction amplifies the interaction between carbon fiber and CO2 molecule for unusually high CO2 uptake and resistive sensing.",1810.06418v1 2020-09-13,Adiabatic theory of SET and RESET transitions,"We develop a phenomenological theory of pulse induced phase transformations behind the SET (from high to low resistive state) and RESET (backward) processes in nonvolatile memory. We show that in modern era devices, both evolve in the adiabatic regime with energy deposition time much shorter than that of thermalization. They are however different by the operating modes: voltage source driven for SET and current source driven for RESET. The characteristic temperatures and transition rates are expressed through material and process parameters.",2009.06057v2 2007-10-29,Thermoelectrical manipulation of nano-magnets,"We propose a device that can operate as a magneto-resistive switch or oscillator. The device is based on a spin-thermo-electronic control of the exchange coupling of two strong ferromagnets through a weakly ferromagnetic spacer. We show that the local Joule heating due to a high concentration of current in a magnetic point contact or a nanopillar can be used to reversibly drive the weak ferromagnet through its Curie point and thereby exchange-decouple the strongly ferromagnetic layers, which have an antiparallel ground state. Such a spin-thermionic parallel-to-antiparallel switching causes magnetoresistance oscillations where the frequency can be controlled by proper biasing from essentially DC to GHz.",0710.5477v1 2007-10-30,Devitrification of a glass-like arrested ferromagnetic phase in La0.5Ca0.5MnO3,"Magnetization measurements in La0.5Ca0.5MnO3 manganite show that the high-temperature long-range ferromagnetic-metallic phase transforms to antiferromagnetic-insulating phase, although a fraction of ferromagnetic-metallic phase undergoes glass-like kinetic arrest and coexists at low temperature with the equilibrium antiferromagnetic-insulating phase. We show here through resistivity measurements that the residual arrested ferromagnetic-metallic fraction can be converted to the equilibrium antiferromagnetic-insulating phase by successive annealing at higher temperatures, possibly through heterogeneous nucleation of equilibrium phase. Significantly, larger fractions of this glassy ferromagnetic-metallic phase can be obtained by cooling in higher fields and larger conversion to equilibrium antiferromagnetic-insulating phase results.",0710.5585v1 2019-03-26,Patterning of diamond with 10 nm resolution by electron-beam-induced etching,"We report on mask-less, high resolution etching of diamond surfaces, featuring sizes down to 10 nm. We use a scanning electron microscope (SEM) together with water vapor, which was injected by a needle directly onto the sample surface. Using this versatile and low-damage technique, trenches with different depths were etched. Cross sections of each trench were obtained by focused ion beam milling and used to calculate the achieved aspect ratios. The developed technique opens up the possibility of mask- and resist-less patterning of diamond for nano-optical and electronic applications.",1903.10824v1 2015-07-11,Insulator/metal phase transition and colossal magnetoresistance in holographic model,"Within massive gravity, we construct a gravity dual for insulator/metal phase transition and colossal magnetoresistance (CMR) effect found in some manganese oxides materials. In heavy graviton limit, a remarkable magnetic-field-sensitive DC resistivity peak appears at the Curie temperature, where an insulator/metal phase transition happens and the magnetoresistance is scaled with the square of field-induced magnetization. We find that metallic and insulating phases coexist below the Curie point and the relation with the electronic phase separation is discussed.",1507.03105v2 2019-10-23,Percolation with plasticity for neuromorphic computing,"We introduce the percolation with plasticity (PWP) systems that exhibit neuromorphic functionalities including multi-valued memory, random number generation, matrix-vector multiplication, and associative learning. PWP systems have multiple (N >> 1) interfaces with external circuitry (electrodes) allowing N! >> 1 measurable interelectrode resistances. Due to the underlying material properties, they undergo successive nonvolatile modifications in response to electric pulses. PWP networks offer some advantages over the existing neural network architectures. Overall, random self-tuning PWP systems with high degree of parallelism, multiple inputs and outputs present close similarities to the cortex of mammalian brain. Understanding their topology, electrodynamics, and statistics opens a field of its own calling upon new theoretical and experimental insights.",1910.10535v1 2019-11-04,Closed-loop electric currents and non-local resistance measurements with wide F/I/N tunnel contacts,"Lateral spin valves are used to generate and characterize pure spin currents. Non-local voltage measured in such structures provides information about spin polarization and spin decay rates. For wide high-transparency F/N contacts it was shown that the Johnson-Silsbee non-local effect is substantially enriched by closed-loop electric currents driven by local spin injection in the electrically dangling part of the valve. For valves with low-transparency F/I/N tunnel contacts such circular currents are strongly suppressed, yet we show that the voltage modifications persist, may be significant, and must be accounted for in the data analysis.",1911.01034v1 2020-01-08,Electrical and optical properties of hydrated amorphous vanadium oxide,"Electrical and optical properties of amorphous vanadium oxide thin films obtained by electrochemical anodic oxidation are studied. It is shown that under cathodic polarization the hydrogen insertion into vanadium oxide from an electrolyte occurs. Metal-insulator transition in amorphous HxVO2 is found to be preserved up to high concentration (x ~ 1.5) of hydrogen. Memory switching with the N-type negative differential resistance, associated with the H+ ionic transfer, is observed in ""V/hydrated amorphous vanadium oxide/Au"" sandwich structures.",2001.02418v1 2020-01-08,Electrical conductivity of vanadium dioxide switching channel,"The electrical conductivity of the switching channel of vanadium dioxide thin-film sandwich structures is studied over a wide temperature range (15-300 K). It is shown that the electrical resistance of the channel varies with temperature as R~exp(aT-b/T) in the high-temperature region (above 70 K). The experimental results are discussed from the viewpoint of the small polaron hopping conduction theory which takes into account the influence of thermal lattice vibrations onto the resonance integral.",2001.03053v1 2021-03-19,Side-leakage of facemask,"Face masks are used to trap particles (or fluid drops) in a porous material (filter) in order to avoid or reduce the transfer of particles between the human lungs (or mouth and nose) and the external environment. The air exchange between the lungs and the environment is assumed to occur through the facemask filter. However, if the resistance to air flow through the filter is high some air (and accompanied particles) will leak through the filter-skin interface. In this paper I will present a model study of the side-leakage problem.",2103.10970v1 2021-04-25,High Pressure RTSC-Hydrides are Extreme Hard Type-II Superconductors,"It is argued that most of the RTSC hydrides are intrinsic hard type-II superconductors with strong pinning effects. The pinning centers are long columnar-like defects, with the radius of the order of the superconducting coherence length. The core and electromagnetic pinning are both equally operative, thus giving maximal pinning potential when vortices are oriented along the columnar axis. The theory predicts: (i) large critical currents, (ii) huge decrease of the temperature broadening of the resistance in magnetic field compared with standard superconductors, (iii) large magnetization hysteresis, (iv) the magnetic irreversible line is pushed toward the second critical field and magnetization relaxation is much slower. That the RTSC-hydrides are hard type-II SC can give rise to new physics in these materials.",2104.12214v1 2022-11-19,A Large-Area RPC Detector for Muography,"A muon telescope equipped with four Resistive Plate Chambers of 2 m$^{2}$ per plane was tested with the muon scattering tomography technique. The telescope was operated during several hours with high atomic number materials located at its center with two detector planes on each side. With an intrinsic efficiency above 98%, spatial resolution around 1 cm and detector planes spaced by 45 cm, it was possible to identify the presence of a 5 cm thick tungsten block in 10 minutes of acquisition. The results obtained after five hours of acquisition are also presented in this communication.",2211.10795v1 2023-05-22,Microcontroller Based AVR Hazardous Gas Detection System using IoT,"MQ-6 Semiconductor Sensor for Combustible Gas detection is a Sensitive Gas sensor. The sensitive material of this MQ-6 gas sensor is SnO2, which works with lower conductivity in clean air. When the target combustible gas exist, the sensors conductivity is higher along with the gas concentration rising. As the conductivity increases the current in the circuit of the sensor increases which results in lower sensor resistance. This change is used to correspond, the output signal of gas concentration. MQ-6 gas sensor has high sensitivity to Methane, Propane and Butane and could be used to detect both Methane and Propane. The sensor could be used to detect different combustible gas especially Methane, it is with low cost and suitable for different application.",2305.12855v1 2017-10-25,High-temperature cyclic oxidation kinetics and microstructural transition mechanisms of Ti-6Al-4V composites reinforced with hybrid (TiC+TiB) networks,"The microstructural features and high-temperature oxidation resistance of hybrid (TiC+TiB) networks reinforced Ti-6Al-4V composites were investigated after fabricated with reaction hot pressing technique. The inhomogeneous distribution of hybrid reinforcers resulted in a sort of stress-induced grain refinement for {\alpha}-Ti matrix phase, which was further facilitated by heterogeneous nucleation upon additive interfaces. HRTEM analyses revealed the crystallographic orientation relation between TiB and alpha-Ti phases as (201)TiB//(-1100)alpha-Ti plus [11-2]//[0001] alpha-Ti, while TiC and {\alpha}-Ti phases maintained the interrelation of (-200)TiC//(-2110) {\alpha}-Ti and [001]TiC//[01-10] alpha-Ti. The hybridly reinforced Ti-6Al-4V/(TiC+TiB) composites displayed superior oxidation resistance to both the sintered matrix alloy and the two composites reinforced solely with TiC or TiB addition during the cyclic oxidation at 873, 973 and 1073 K respectively for 100 h. The hybrid reinforcers volume fraction was a more influential factor to improve oxidation resistance than the matrix alloy powder size. As temperature rose from 873 to 1073 K, the oxidation kinetics transferred from the nearly parabolic type through qusilinear tendency into the finally linear mode. This corresponded to the morphological transition of oxide scales from a continuous protective film to a partially damaged layer and ended up with the complete spallation of alternating alumina and rutile multilayers. A phenomenological model was proposed to elucidate the growth process of oxides scales. The release of thermal stress, the suppression of oxygen diffusion and the fastening of oxide adherence were found as the three major mechanisms to enhance the oxidation resistance of hybrid reinforced composites.",1710.09315v1 2007-07-20,A mechanism for unipolar resistance switching in oxide non-volatile memory devices,"Building on a recently introduced model for non-volatile resistive switching, we propose a mechanism for unipolar resistance switching in metal-insulator-metal sandwich structures. The commutation from the high to low resistance state and back can be achieved with successive voltage sweeps of the same polarity. Electronic correlation effects at the metal-insulator interface are found to play a key role to produce a resistive commutation effect in qualitative agreement with recent experimental reports on binary transition metal oxide based sandwich structures.",0707.3077v1 2013-08-02,Precision Quantum Hall Resistance Measurement on Epitaxial Graphene Device in Low Magnetic Field,"Precision quantum Hall resistance (QHR) measurements were performed on large-area epitaxial graphene device at low magnetic fields (B = 2 T - 8 T) at temperature T = 1.5 K. Hall resistance was measured using Cryogenic Current Comparator resistance bridge with high biasing current Isd = 40 micro ampere. The results showed that at B = 8 T the relative deviation of Hall resistance from the expected quantized value h/2e2 is within experimental uncertainty of 3.5 parts in 108 and remained below 0.35 parts per million (ppm) down to B = 3 T.",1308.0456v1 2011-01-30,Spin transport in magnetically ordered systems: effect of the lattice relaxation time,"Spin resistivity $R$ has been shown to result mainly from the scattering of itinerant spins with magnetic impurities and lattice spins. $R$ is proportional to the spin-spin correlation so that its behavior is very complicated near and at the magnetic phase transition of the lattice spins. For the time being there are many new experimental data on the spin resistivity going from semiconductors to superconductors. Depending on materials, various behaviors have been observed. There is however no theory so far which gives a unified mechanism for spin resistivity in magnetic materials. Recently, we have showed Monte Carlo results for different systems. We found that the spin resistivity is very different from one material to another. In this paper, we show for the first time how the dynamic relaxation time of the lattice spins affects the resistivity of itinerant spins observed in Monte Carlo simulation.",1101.5789v1 2020-09-16,Resistive switching in reverse: voltage driven formation of a transverse insulating barrier,"Application of an electric stimulus to a material with a metal-insulator transition can trigger a large resistance change. Resistive switching from an insulating into a metallic phase, which typically occurs by the formation of conducting filaments parallel to the current flow, has been an active research topic. Here we present the discovery of an opposite, metal-to-insulator switching that proceeds via nucleation and growth of an insulating barrier perpendicular to the driving current. The barrier formation leads to an unusual N-type negative differential resistance in the current-voltage characteristics. Electrically inducing a transverse barrier enables a novel approach to voltage-controlled magnetism. By triggering a metal-to-insulator resistive switching in a magnetic material, local on/off control of ferromagnetism can be achieved by a global voltage bias applied to the whole device.",2009.07412v1 2021-08-14,Voltage-controlled magnetism enabled by resistive switching,"The discovery of new mechanisms of controlling magnetic properties by electric fields or currents furthers the fundamental understanding of magnetism and has important implications for practical use. Here, we present a novel approach of utilizing resistive switching to control magnetic anisotropy. We study a ferromagnetic oxide that exhibits an electrically triggered metal-to-insulator phase transition producing a volatile resistive switching. This switching occurs in a characteristic spatial pattern: the formation of a transverse insulating barrier inside a metallic matrix resulting in an unusual ferromagnetic/paramagnetic/ferromagnetic configuration. We found that the formation of this voltage-driven paramagnetic insulating barrier is accompanied by the emergence of a strong uniaxial magnetic anisotropy that overpowers the intrinsic material anisotropy. Our results demonstrate that resistive switching is an effective tool for manipulating magnetic properties. Because resistive switching can be induced in a very broad range of materials, our findings could enable a new class of voltage-controlled magnetism systems.",2108.06445v1 2022-08-02,Investigating thermal transport in knotted graphene nanoribbons using non-equilibrium molecular dynamics,"In this work, we investigated the effect of knots in the thermal transport of graphene nanoribbons through non-equilibrium molecular dynamics simulations. We considered the cases of one, two, and three knots are present. Temperature jumps appear in the temperature profile where the knots are located, which indicates that they introduce thermal resistances in the system, similar to interfacial Kapitza resistance present between two different materials and/or single materials with defects and/or lattice distortions. We found that the thermal resistance introduced by each individual knot is essentially the same as the overall resistance increase linearly with the number of knots, as they behave as thermal resistances associated in series. Also, the relative position between each knot in the arrangement does not strongly affect the thermal current produced by the temperature gradient, showing a weak thermal rectification effect.",2208.01751v1 2010-05-21,Effect of Heterogeneous Mixing and Vaccination on the Dynamics of Anthelmintic Resistance: A Nested Model,"Anthelmintic resistance is a major threat to current measures for helminth control in humans and animals. The introduction of anthelmintic vaccines, as a complement to or replacement for drug treatments, has been advocated as a preventive measure. Here, a computer-based simulation, tracking the dynamics of hosts, parasites and parasite-genes, shows that, depending on the degree of host-population mixing, the frequency of totally recessive autosomes associated with anthelmintic resistance can follow either a fast dynamical regime with a low equilibrium point or a slow dynamical regime with a high equilibrium point. For fully dominant autosomes, only one regime is predicted. The effectiveness of anthelminthic vaccines against resistance is shown to be strongly influenced by the underlying dynamics of resistant autosomes. Vaccines targeting adult parasites, by decreasing helminth fecundity or lifespan, are predicted to be more effective than vaccines targeting parasite larvae, by decreasing host susceptibility to infection, in reducing the spread of resistance. These results may inform new strategies to prevent, monitor and control the spread of anthelmintic resistance, including the development of viable anthelmintic vaccines.",1005.3891v1 2018-06-20,Modeling continuous levels of resistance to multidrug therapy in cancer,"Multidrug resistance consists of a series of genetic and epigenetic alternations that involve multifactorial and complex processes, which are a challenge to successful cancer treatments. Accompanied by advances in biotechnology and high-dimensional data analysis techniques that are bringing in new opportunities in modeling biological systems with continuous phenotypic structured models, we study a cancer cell population model that considers a multi-dimensional continuous resistance trait to multiple drugs to investigate multidrug resistance. We compare our continuous resistance trait model with classical models that assume a discrete resistance state and classify the cases when the continuum and discrete models yield different dynamical patterns in the emerging heterogeneity in response to drugs. We also compute the maximal fitness resistance trait for various continuum models and study the effect of epimutations. Finally, we demonstrate how our approach can be used to study tumor growth regarding the turnover rate and the proliferating fraction, and show that a continuous resistance level may result in a different dynamics when compared with the predictions of other discrete models.",1806.07557v1 2021-01-18,Hubs-biased resistance distances on graphs and networks,"We define and study two new kinds of ""effective resistances"" based on hubs-biased -- hubs-repelling and hubs-attracting -- models of navigating a graph/network. We prove that these effective resistances are squared Euclidean distances between the vertices of a graph. They can be expressed in terms of the Moore-Penrose pseudoinverse of the hubs-biased Laplacian matrices of the graph. We define the analogous of the Kirchhoff indices of the graph based of these resistance distances. We prove several results for the new resistance distances and the Kirchhoff indices based on spectral properties of the corresponding Laplacians. After an intensive computational search we conjecture that the Kirchhoff index based on the hubs-repelling resistance distance is not smaller than that based on the standard resistance distance, and that the last is not smaller than the one based on the hubs-attracting resistance distance. We also observe that in real-world brain and neural systems the efficiency of standard random walk processes is as high as that of hubs-attracting schemes. On the contrary, infrastructures and modular software networks seem to be designed to be navigated by using their hubs.",2101.07103v2 2021-10-18,Low-Frequency 1/f Noise Characteristics of Ultra-Thin AlO$_{x}$-Based Resistive Switching Memory Devices with Magneto-Resistive Responses,"Low-frequency 1/f voltage noise has been employed to probe stochastic charge dynamics in AlO$_{x}$-based non-volatile resistive memory devices exhibiting both resistive switching (RS) and magneto-resistive (MR) effects. A 1/f$^{\gamma}$ noise power spectral density is observed in a wide range of applied voltage biases. By analyzing the experimental data within the framework of Hooge's empirical relation, we found that the Hooge's parameter $\alpha$ and the exponent $\gamma$ exhibit a distinct variation upon the resistance transition from the low resistance state (LRS) to the high resistance state (HRS), providing strong evidence that the electron trapping/de-trapping process, along with the electric field-driven oxygen vacancy migration in the AlO$_x$ barrier, plays an essential role in the charge transport dynamics of AlO$_x$-based RS memory devices.",2110.09331v1 2023-07-24,Clustering MIC data through Bayesian mixture models: an application to detect M. Tuberculosis resistance mutations,"Antimicrobial resistance is becoming a major threat to public health throughout the world. Researchers are attempting to contrast it by developing both new antibiotics and patient-specific treatments. In the second case, whole-genome sequencing has had a huge impact in two ways: first, it is becoming cheaper and faster to perform whole-genome sequencing, and this makes it competitive with respect to standard phenotypic tests; second, it is possible to statistically associate the phenotypic patterns of resistance to specific mutations in the genome. Therefore, it is now possible to develop catalogues of genomic variants associated with resistance to specific antibiotics, in order to improve prediction of resistance and suggest treatments. It is essential to have robust methods for identifying mutations associated to resistance and continuously updating the available catalogues. This work proposes a general method to study minimal inhibitory concentration (MIC) distributions and to identify clusters of strains showing different levels of resistance to antimicrobials. Once the clusters are identified and strains allocated to each of them, it is possible to perform regression method to identify with high statistical power the mutations associated with resistance. The method is applied to a new 96-well microtiter plate used for testing M. Tuberculosis.",2307.12603v1 2023-06-19,On the Active Components in Crystalline Li-Nb-O and Li-Ta-O Coatings from First Principles,"Layered-oxide $\mathrm{LiNi_xMn_yCo_{1-x-y}O_2}$ (NMC) positive electrodes with high Nickel content, deliver high voltages and energy densities. However, a high nickel content, e.g., $x$ = 0.8 (NMC 811), can lead to high surface reactivity, which can trigger thermal runaway and gas generation. While claimed safer, all-solid-state batteries still suffer from high interfacial resistance. Here, we investigate niobate and tantalate coating materials, which can mitigate the interfacial reactivities in Li-ion and all-solid-state batteries. First-principles calculations reveal the multiphasic nature of Li-Nb-O and Li-Ta-O coatings, containing mixtures of $\mathrm{LiNbO_3}$ and $\mathrm{Li_3NbO_4}$, or of $\mathrm{LiTaO_3}$ and $\mathrm{Li_3TaO_4}$. The concurrence of several phases in Li-Nb-O or Li-Ta-O modulates the type of stable native defects in these coatings. Li-Nb-O and Li-Ta-O coating materials can form favorably lithium vacancies $\mathrm{Vac^{'}_{Li}}$ and antisite defects $\mathrm{Nb^{\bullet \bullet \bullet \bullet}_{Li}}$ ($\mathrm{Ta^{\bullet \bullet \bullet \bullet}_{Li}}$) combined into charge-neutral defect complexes. Even in defective crystalline $\mathrm{LiNbO_3}$ (or $\mathrm{LiTaO_3}$), we reveal poor Li-ion conduction properties. In contrast, $\mathrm{Li_3NbO_4}$ and $\mathrm{Li_3TaO_4}$ that are introduced by high-temperature calcinations can provide adequate Li-ion transport in these coatings. Our in-depth investigation of the structure-property relationships in the important Li-Nb-O and Li-Ta-O coating materials helps to develop more suitable calcination protocols to maximize the functional properties of these niobates and tantalates.",2306.10716v1 2020-01-23,Large Enhancement of Thermoelectric Efficiency Due to a Pressure-Induced Lifshitz Transition in SnSe,"Lifshitz transition, a change in Fermi surface topology, is likely to greatly influence exotic correlated phenomena in solids, such as high-temperature superconductivity and complex magnetism. However, since the observation of Fermi surfaces is generally difficult in the strongly correlated systems, a direct link between the Lifshitz transition and quantum phenomena has been elusive so far. Here, we report a marked impact of the pressure-induced Lifshitz transition on thermoelectric performance for SnSe, a promising thermoelectric material without strong electron correlation. By applying pressure up to 1.6 GPa, we have observed a large enhancement of thermoelectric power factor by more than 100% over a wide temperature range (10-300 K). Furthermore, the high carrier mobility enables the detection of quantum oscillations of resistivity, revealing the emergence of new Fermi pockets at ~0.86 GPa. The observed thermoelectric properties linked to the multi-valley band structure are quantitatively reproduced by first-principles calculations, providing novel insight into designing the SnSe-related materials for potential valleytronic as well as thermoelectric applications.",2001.08674v1 2009-07-10,Cellulose-Bound Magnesium Diboride Superconductivity,"Two-phase superconductor tapes were produced by blending high purity magnesium diboride powder with a liquid ethylcellulose-based polymeric binder. This procedure produced a material which is easily formable with a high superconducting transition temperature (38K). We show that the bulk superconducting properties are not affected by the presence of the binder, nor is there any evidence of a chemical reaction between the superconducting particles and the binder. However, the transport properties of the material are strongly affected by the presence of the binder, which leads to a seven order of magnitude increase of the normal state resistance along with a seven order of magnitude decrease of the transport critical current density. This new material is shown to be equivalent to a system of coupled Josephson junctions.",0907.1744v1 2010-06-27,Soft capacitor fibers using conductive polymers for electronic textiles,"A novel, highly flexible, conductive polymer-based fiber with high electric capacitance is reported. In its crossection the fiber features a periodic sequence of hundreds of conductive and isolating plastic layers positioned around metallic electrodes. The fiber is fabricated using fiber drawing method, where a multi-material macroscopic preform is drawn into a sub-millimeter capacitor fiber in a single fabrication step. Several kilometres of fibers can be obtained from a single preform with fiber diameters ranging between 500um -1000um. A typical measured capacitance of our fibers is 60-100 nF/m and it is independent of the fiber diameter. For comparison, a coaxial cable of the comparable dimensions would have only ~0.06nF/m capacitance. Analysis of the fiber frequency response shows that in its simplest interrogation mode the capacitor fiber has a transverse resistance of 5 kOhm/L, which is inversely proportional to the fiber length L and is independent of the fiber diameter. Softness of the fiber materials, absence of liquid electrolyte in the fiber structure, ease of scalability to large production volumes, and high capacitance of our fibers make them interesting for various smart textile applications ranging from distributed sensing to energy storage.",1006.5221v1 2015-03-06,Conductivity of a Weyl semimetal with donor and acceptor impurities,"We study transport in a Weyl semimetal with donor and acceptor impurities. At sufficiently high temperatures transport is dominated by electron-electron interactions, while the low-temperature resistivity comes from the scattering of quasiparticles on screened impurities. Using the diagrammatic technique, we calculate the conductivity $\sigma(T,\omega,n_A,n_D)$ in the impurities-dominated regime as a function of temperature $T$, frequency $\omega$, and the concentrations $n_A$ and $n_D$ of donors and acceptors and discuss the crossover behaviour between the regimes of low and high temperatures and impurity concentrations. In a sufficiently compensated material [$|n_A-n_D|\ll(n_A+n_D)$] with a small effective fine structure constant $\alpha$, $\sigma(\omega,T)\propto T^2/(T^{-2}-i\omega\cdot\text{const})$ in a wide interval of temperatures. For very low temperatures or in the case of an uncompensated material the transport is effectively metallic. We discuss experimental conditions necessary for realising each regime.",1503.02078v2 2015-10-31,High-performance Thermal Interface Material Based on Few-layer Graphene Composite,"We developed high-performance thermal interface materials (TIMs) based on few-layer graphene (FLG) composite, where FLG was prepared by the interlayer catalytic exfoliation (ICE) method. We experimentally demonstrated feasibility of FLG composites as TIMs by investigating their thermal and mechanical properties, and reliability. We measured the thermal interface resistance ($R_{int}$) between FLG composite TIMs (FLGTs) and copper and to be 3.2$\pm$1.7 and 4.3$\pm$1.4 $mm^2$K/W for 5 vol.% and 10 vol.% FLGTs at 330 K, respectively, comparable to or even lower than that of many commercial TIMs. In addition, the thermal conductivity ($\kappa_{TIM}$) of FLGTs is increased by an enhancement factor ($\beta$) of ~17 as the FLG concentration increases from 0 to 10 vol.%. We also characterized Vickers hardness and glass transition temperature ($T_g$) of our FLGTs. We find that our FLGTs are thermally and mechanically reliable within practical operating temperature and pressure ranges.",1511.00076v2 2016-02-16,Perfect charge compensation in extremely large magnetoresistance materials LaSb and LaBi revealed by the first-principles calculations,"By the first-principles electronic structure calculations, we have systematically studied the electronic structures of recently discovered extremely large magnetoresistance (XMR) materials LaSb and LaBi. We find that both LaSb and LaBi are semimetals with the electron and hole carriers in perfect balance. The calculated carrier densities in the order of $10^{20}$ cm$^{-3}$ are in good agreement with the experimental values, implying long mean free time of carriers and thus high carrier mobilities. With a semiclassical two-band model, the perfect charge compensation and high carrier mobilities naturally explain (i) the XMR observed in LaSb and LaBi; (ii) the non-saturating quadratic dependence of XMR on external magnetic field; and (iii) the resistivity plateau in the turn-on temperature behavior at very low temperatures. The explanation of these features without resorting to the topological effect indicates that they should be the common characteristics of all perfectly electron-hole compensated semimetals.",1602.05061v1 2016-06-17,"Homogeneously bright, flexible and foldable lighting devices with functionalised graphene electrodes","Alternating current electroluminescent technology allows the fabrication of large area, flat and flexible lights. Presently the maximum size of a continuous panel is limited by the high resistivity of available transparent electrode materials causing a visible gradient of brightness. Here, we demonstrate that the use of the best known transparent conductor FeCl$_{3}$-intercalated few-layer graphene boosts the brightness of electroluminescent devices by 49$\%$ compared to pristine graphene. Intensity gradients observed for high aspect ratio devices are undetectable when using these highly conductive electrodes. Flat lights on polymer substrates are found to be resilient to repeated and flexural strains.",1606.05482v1 2017-10-27,The Quantum Hall Effect with Wilczek's charged magnetic flux tubes instead of electrons,"Composites formed from charged particles and magnetic flux tubes, proposed by Wilczek, are one model for anyons - particles obeying fractional statistics. Here we propose a scheme for realizing charged flux tubes, in which a charged object with an intrinsic magnetic dipole moment is placed between two semi-infinite blocks of a high permeability ($\mu_r$) material, and the images of the magnetic moment create an effective flux tube. We show that the scheme can lead to a realization of Wilczek's anyons, when a two-dimensional electron system, which exhibits the integer quantum Hall effect (IQHE), is sandwiched between two blocks of the high-$\mu_r$ material with a temporally fast response (in the cyclotron and Larmor frequency range). The signature of Wilczek's anyons is a slight shift of the resistivity at the plateau of the IQHE. Thus, the quest for high-$\mu_r$ materials at high frequencies, which is underway in the field of metamaterials, and the quest for anyons, are here found to be on the same avenue.",1710.10108v2 2020-03-03,Chemical sensing with atomically-thin metals templated by a two-dimensional insulator,"Boosting the sensitivity of solid-state gas sensors by incorporating nanostructured materials as the active sensing element can be complicated by interfacial effects. Interfaces at nanoparticles, grains, or contacts may result in non-linear current-voltage response, high electrical resistance, and ultimately, electric noise that limits the sensor read-out. Here we report the possibility to prepare nominally one atom thin, electrically continuous metals, by straightforward physical vapor deposition on the carbon zero-layer grown epitaxially on silicon carbide. With platinum as the metal, its electrical conductivity is strongly modulated when interacting with chemical analytes, due to charges being transferred to/from Pt. This, together with the scalability of the material, allows us to microfabricate chemiresistor devices for electrical read-out of chemical species with sub part-per-billion detection limits. The two-dimensional system formed by atomically-thin metals open up a route for resilient and high sensitivity chemical detection, and could be the path for designing new heterogeneous catalysts with superior activity and selectivity.",2003.01594v1 2020-04-27,Runaway dynamics in the DT phase of ITER operations in the presence of massive material injection,"A runaway avalanche can result in a conversion of the initial plasma current into a relativistic electron beam in high current tokamak disruptions. We investigate the effect of massive material injection of deuterium-noble gas mixtures on the coupled dynamics of runaway generation, resistive diffusion of the electric field, and temperature evolution during disruptions in the DT phase of ITER operations. We explore the dynamics over a wide range of injected concentrations and find substantial runaway currents, unless the current quench time is intolerably long. The reason is that the cooling associated with the injected material leads to high induced electric fields that, in combination with a significant recombination of hydrogen isotopes, leads to a large avalanche generation. Balancing Ohmic heating and radiation losses provides qualitative insights into the dynamics, however, an accurate modeling of the temperature evolution based on energy balance appears crucial for quantitative predictions.",2004.12861v3 2020-09-04,Magnon-induced Giant Anomalous Nernst Effect in Single Crystal MnBi,"Thermoelectric modules are a promising approach to energy harvesting and efficient cooling. In addition to the longitudinal Seebeck effect, recently transverse devices utilizing the anomalous Nernst effect (ANE) have attracted interest. For high conversion efficiency, it is required that the material should have a large ANE thermoelectric power and low electrical resistance, the product of which is the ANE conductivity. ANE is usually explained in terms of intrinsic contributions from Berry curvature. Our observations suggest that extrinsic contributions also matter. Studying single-crystal MnBi, we find a very high ANE thermopower (~10 $\mu$V/K) under 0.6 T at 80 K, and a transverse thermoelectric conductivity of over 40 A/Km. With insight from theoretical calculations, we attribute this large ANE predominantly to a new advective magnon contribution arising from magnon-electron spin-angular momentum transfer. We propose that introducing large spin-orbit coupling into ferromagnetic materials may enhance the ANE through the extrinsic contribution of magnons.",2009.02211v3 2022-02-10,Nanostructured transition metal dichalcogenide multilayers for advanced nanophotonics,"Transition metal dichalcogenides (TMDs) attract significant attention due to their exceptional optical, excitonic, mechanical, and electronic properties. Nanostructured multilayer TMDs were recently shown to be highly promising for nanophotonic applications, as motivated by their exceptionally high refractive indexes and optical anisotropy. Here, we extend this vision to more sophisticated structures, such as periodic arrays of nanodisks and nanoholes, as well as proof-of-concept waveguides and resonators. We specifically focus on various advanced nanofabrication strategies, including careful selection of resists for electron beam lithography and etching methods. The specific materials studied here include semiconducting WS$_2$, in-plane anisotropic ReS$_2$, and metallic TaSe$_2$, TaS$_2$ and NbSe$_2$. The resulting nanostructures can potentially impact several nanophotonic and optoelectronic areas, including high-index nanophotonics, plasmonics and on-chip optical circuits. The knowledge of TMD material-dependent nanofabrication parameters developed here will help broaden the scope of future applications of these materials in all-TMD nanophotonics.",2202.04898v1 2021-01-20,Electrically-Insulating Flexible Films with Quasi-One-Dimensional van-der-Waals Fillers as Efficient Electromagnetic Shields,"We report polymer composite films containing fillers comprised of quasi-one-dimensional (1D) van der Waals materials, specifically transition metal trichalcogenides containing 1D structural motifs that enable their exfoliation into bundles of atomic threads. These nanostructures are characterized by extremely large aspect ratios of up to 10^6. The polymer composites with low loadings of quasi-1D TaSe3 fillers (below 3 vol. %) revealed excellent electromagnetic interference shielding in the X-band GHz and EHF sub-THz frequency ranges, while remaining DC electrically insulating. The unique electromagnetic shielding characteristics of these films are attributed to effective coupling of the electromagnetic waves to the high-aspect-ratio electrically-conductive TaSe3 atomic-thread bundles even when the filler concentration is below the electrical percolation threshold. These novel films are promising for high-frequency communication technologies, which require electromagnetic shielding films that are flexible, lightweight, corrosion resistant, electrically insulating and inexpensive.",2101.08239v1 2020-05-07,Understanding cooperative loading in carbon nanotube fibres through in-situ structural studies during stretching,"Carbon nanotube (CNT) fibres are firmly established as a new high-performance fibre, but their tensile mechanical properties remain a relatively small fraction of those of the constituent CNTs. Clear structure-property relations and accurate mechanical models are pressing requirements to bridge this gap. In this work we analyse the structural evolution and molecular stress transfer in CNT fibres by performing in-situ synchrotron wide- and small-angle X-ray scattering and Raman spectroscopy during tensile deformation. The results show that CNT fibres can be accurately described as network of bundles that slide progressively according to the initial orientation distribution function of the material following a Weibull distribution. This model decouples the effects of CNT alignment and degree of cooperative loading, as demonstrated for fibres produced at different draw ratios. It also helps explain the unusually high toughness (fracture energy) of CNT fibres produced by the direct spinning method, a key property for impact resistance in structural materials, for example.",2005.03305v2 2020-12-02,Crystallographic Reconstruction Driven Modified Mechanical Properties in Anisotropic Rhenium Disulfides,"Atomic-scale investigation on mechanical behaviors is highly necessary to fully understand the fracture mechanics especially of brittle materials, which are determined by atomic-scale phenomena (e.g., lattice trapping). Here, exfoliated anisotropic rhenium disulfide (ReS2) flakes are used to investigate atomic-scale crack propagation depending on the propagation directions. While the conventional strain-stress curves exhibit a strong anisotropy depending on the cleavage direction of ReS2, but our experimental results show a reduced cleavage anisotropy due to the lattice reconstruction in [100] cracking with high resistance to fracture. In other words, [010] and [110] cracks with low barriers to cleavage exhibit the ultimate sharpness of the crack tip without plastic deformation, whereas [100] cracks drive lattice rotation on one side of the crack, leading to a non-flat grain boundary formation. Finally, crystallographic reconstruction associated with the high lattice randomness of two-dimensional materials drives to a modified cleavage tendency, further indicating the importance of atomic-scale studies for a complete understanding of the mechanics.",2012.01045v1 2021-03-04,Observation of an Unusual Colossal Anisotropic Magnetoresistance Effect in an Antiferromagnetic Semiconductor,"Searching for novel antiferromagnetic materials with large magnetotransport response is highly demanded for constructing future spintronic devices with high stability, fast switching speed, and high density. Here we report a colossal anisotropic magnetoresistance effect in an antiferromagnetic binary compound with layered structure rare-earth dichalcogenide EuTe2. The AMR reaches 40000%, which is 4 orders of magnitude larger than that in conventional antiferromagnetic alloys. Combined magnetization, resistivity, and theoretical analysis reveal that the colossal AMR effect is attributed to a novel mechanism of vector-field tunable band structure, rather than the conventional spin-orbit coupling mechanism. Moreover, it is revealed that the strong hybridization between orbitals of Eu-layer with localized spin and Te-layer with itinerant carriers is extremely important for the large AMR effect. Our results suggest a new direction towards exploring AFM materials with prominent magnetotransport properties, which creates an unprecedented opportunity for AFM spintronics applications.",2103.02818v1 2023-01-17,Comparing Methods of Characterizing Energetic Disorder in Organic Solar Cells,"Energetic disorder has been known for decades to limit the performance of structurally disordered semiconductors such as amorphous silicon and organic semiconductors. However, in the past years, high performance organic solar cells have emerged showing a continuously reduced amount of energetic disorder. While searching for future high efficiency material systems, it is therefore important to correctly characterize this energetic disorder. While there are several techniques in literature, the most common approaches to probe the density of defect states are using optical excitation as in external quantum efficiency measurements or sequential filling of the tail states by applying an external voltage as in admittance spectroscopy. A metanalysis of available literature as well as our experiments using four characterization techniques on two material systems reveal that electrical, voltage-dependent measurements frequently yield higher values of energetic disorder than optical measurements. With drift-diffusion simulations, we demonstrate that the approaches probe different energy ranges of the subband-gap density of states. We further explore the limitations of the techniques and find that extraction of information from a capacitance-voltage curve can be inhibited by an internal series resistance. Thereby, we explain the discrepancies between measurements techniques with sensitivity to different energy ranges and electronic parameters.",2301.06792v1 2023-06-12,Significant improvement of the lower critical field in Y doped Nb: potential replacement of basic material for the radio-frequency superconducting cavity,"The research of high energy and nuclear physics requires high power accelerators, and the superconducting radio-frequency (SRF) cavity is regarded as their engine. Up to now, the widely used practical and effective material for making the SRF cavity is pure Nb. The key parameter that governs the efficiency and the accelerating field (E_acc) of a SRF cavity is the lower critical field Hc1. Here, we report a significant improvement of Hc1 for a new type of alloy, Nb_{1-x}Y_x fabricated by the arc melting technique. Experimental investigations with multiple tools including x-ray diffraction, scanning electron microscopy, resistivity and magnetization are carried out, showing that the samples have good quality and a 30%-60% enhancement of Hc1. First principle calculations indicate that this improvement is induced by the delicate tuning of a Lifshitz transition of a Nb derivative band near the Fermi energy, which increases the Ginzburg-Landau parameter and Hc1. Our results may trigger a replacement of the basic material and thus a potential revolution for manufacturing the SRF cavity.",2306.06915v1 2023-07-18,Observation of giant two-level systems in a granular superconductor,"Disordered thin films are a common choice of material for superconducting, high impedance circuits used in quantum information or particle detector physics. A wide selection of materials with different levels of granularity are available, but, despite low microwave losses being reported for some, the high degree of disorder always implies the presence of intrinsic defects. Prominently, quantum circuits are prone to interact with two-level systems (TLS), typically originating from solid state defects in the dielectric parts of the circuit, like surface oxides or tunneling barriers. We present an experimental investigation of TLS in granular aluminum thin films under applied mechanical strain and electric fields. The analysis reveals a class of strongly coupled TLS having electric dipole moments up to 30 eA, an order of magnitude larger than dipole moments commonly reported for solid state defects. Notably, these large dipole moments appear more often in films with a higher resistivity. Our observations shed new light on granular superconductors and may have implications for their usage as a quantum circuit material.",2307.09078v2 2024-03-01,First-principles Investigation of Thermodynamic Properties of CrNbO4 and CrTaO4,"In the present study, the DFT+U method was employed to predict the thermodynamic properties of Cr2O3, Nb2O5, and Ta2O5. Results were benchmarked with experimental data showing high accuracy, except for the negative thermal expansion (NTE) of Nb2O5, which is attributed to its polymorphic complexity. Additionally, we extended our analysis to rutile-type oxides CrNbO4 and CrTaO4, examining their entropy and heat capacity at finite temperatures. CrNbO4 displayed slightly higher entropy and heat capacity at high temperatures. The mean linear thermal expansion coefficients for CrNbO4 and CrTaO4 from 500 K to 2000 K were predicted to be 6.00*10-6/K and 13.49*10-6/K, respectively, corroborating with DFT predictions and experimental evidence. Our research highlights the precision of the DFT+U and phonon methods in predicting the thermodynamic properties of oxide materials, offering insights into the design of corrosion-resistant materials.",2403.00705v1 2017-03-05,Response to Comment on 'Spin-Orbit Logic with Magnetoelectric Nodes: A Scalable Charge Mediated Nonvolatile Spintronic Logic' (arXiv:1607.06690),"In this technical note, we address the comments on the energy estimates for Magnetoelectric Spin-orbit (MESO) Logic, a new logic device proposed by the authors. We provide an analytical derivation of the switching energy, and support it with time-domain circuit simulations using a self-consistent ferroelectric (FE) compact model. While the energy to charge a capacitor is dissipated in the interconnect and transistor resistance, we note that the energy to switch a capacitor and a FE is independent of the interconnect resistance value to the first order. Also device design can mitigate the parasitic energy losses. We further show the circuit simulations for a sub 10 aJ switching operation of a MESO logic device comprehending: a) Energy stored in multiferroic; b) Energy dissipation in the resistance of the interconnect, Ric ; c) Energy dissipation in the inverse spin-orbit coupling (ISOC) spin to charge converter Risoc; d) Supply, ground resistance, and transistor losses. We also identify the requirements for the resistivity of the spin-orbit coupling materials and address the effect of internal resistance of the spin to charge conversion layer. We provide the material parameter space where MESO (with a fan-out of 1 and interconnect) achieves sub 10 aJ switching energy with path for scaling via ferroelectric/magnetoelectric/spin-orbit materials development.",1703.01559v1 2014-11-05,Modeling of High Composition AlGaN Channel HEMTs with Large Threshold Voltage,"We report on the potential of high electron mobility transistors (HEMTs) consisting of high composition AlGaN channel and barrier layers for power switching applications. Detailed 2D simulations show that threshold voltages in excess of 3 V can be achieved through the use of AlGaN channel layers. We also calculate the two-dimensional electron gas (2DEG) mobility in AlGaN channel HEMTs and evaluate their power figures of merit as a function of device operating temperature and Al mole fraction in the channel. Our models show that power switching transistors with AlGaN channels would have comparable on-resistance to GaN-channel based transistors for the same operation voltage. The modeling in this paper shows the potential of high composition AlGaN as a channel material for future high threshold enhancement mode transistors.",1411.1447v1 2016-11-10,Ultra-high vacuum compatible preparation chain for intermetallic compounds,"We report the development of a versatile material preparation chain for intermetallic compounds that focuses on the realization of a high-purity growth environment. The preparation chain comprises of an argon glovebox, an inductively heated horizontal cold boat furnace, an arc melting furnace, an inductively heated rod casting furnace, an optically heated floating-zone furnace, a resistively heated annealing furnace, and an inductively heated annealing furnace. The cold boat furnace and the arc melting furnace may be loaded from the glovebox by means of a load-lock permitting to synthesize compounds starting with air-sensitive elements while handling the constituents exclusively in an inert gas atmosphere. All furnaces are all-metal sealed, bakeable, and may be pumped to ultra-high vacuum. We find that the latter represents an important prerequisite for handling compounds with high vapor pressure under high-purity argon atmosphere. We illustrate operational aspects of the preparation chain in terms of the single-crystal growth of the heavy-fermion compound CeNi2Ge2.",1611.03392v1 2020-08-06,Granular superconductors for high kinetic inductance and low loss quantum devices,"Granular aluminum is a promising material for high kinetic inductance devices such as qubit circuits. It has the advantage over atomically disordered materials such as NbN_x, to maintain a high kinetic inductance concomitantly with a high quality factor. We show that high quality nano-scale granular aluminum films having a sharp superconducting transition with normal state resistivity values of the order of 1x10^5 \mu\Omega cm and kinetic inductance values of the order of 10 nH/sq can be obtained, surpassing state of the art values. We argue that this is a result of the different nature of the metal-to-insulator transition, being electronic correlations driven (Mott type) in the former and disorder driven (Anderson type) in the latter.",2008.02860v1 2023-11-14,A calculation method to estimate thermal conductivity of high entropy ceramic for thermal barrier coatings,"High entropy ceramics are highly promising as next generation thermal barrier coatings due to their unique disorder structure, which imparts ultra-low thermal conductivity and good high temperature stability. Unlike traditional ceramic materials, the thermal resistance in high entropy ceramics predominantly arises from phonon-disorder scattering rather than phonon-phonon interactions. In this study, we propose a calculation method based on the supercell phonon unfolding (SPU) technique to predict the thermal conductivity of high entropy ceramics, specially focusing on rocksalt oxides structures. Our prediction method relies on using the reciprocal value of SPU phonon spectra linewidth as an indicator of phonon lifetime. The obtained results demonstrate a strong agreement between the predicted thermal conductivities and the experimental measurements, validating the feasibility of our calculation method. Furthermore, we extensively investigate and discuss the atomic relaxation and lattice distortion effects in 5-dopants and 6-dopants rocksalt structures during the process.",2311.08246v1 2022-04-14,Non-equilibrium Phonon Thermal Resistance at MoS2/Oxide and Graphene/Oxide Interfaces,"Accurate measurements and physical understanding of thermal boundary resistance (R) of two-dimensional (2D) materials are imperative for effective thermal management of 2D electronics and photonics. In previous studies, heat dissipation from 2D material devices was presumed to be dominated by phonon transport across the interfaces. In this study, we find that in addition to phonon transport, thermal resistance between non-equilibrium phonons in the 2D materials could play a critical role too when the 2D material devices are internally self-heated, either optically or electrically. We accurately measure R of oxide/MoS2/oxide and oxide/graphene/oxide interfaces for three oxides (SiO2, HfO2, Al2O3) by differential time-domain thermoreflectance (TDTR). Our measurements of R across these interfaces with external heating are 2-to-4 times lower than previously reported R of the similar interfaces measured by Raman thermometry with internal self-heating. Using a simple model, we show that the observed discrepancy can be explained by an additional internal thermal resistance (Rint) between non-equilibrium phonons present during Raman measurements. We subsequently estimate that for MoS2 and graphene, Rint is about 31 and 22 m2 K/GW, respectively. The values are comparable to the thermal resistance due to finite phonon transmission across interfaces of 2D materials and thus cannot be ignored in the design of 2D material devices. Moreover, the non-equilibrium phonons also lead to a different temperature dependence than that by phonon transport. As such, our work provides important insights into physical understanding of heat dissipation in 2D material devices.",2204.06975v1 1996-08-24,Band Structure and Transport Properties of CrO_2,"Local Spin Density Approximation (LSDA) is used to calculate the energy bands of both the ferromagnetic and paramagnetic phases of metallic CrO_2. The Fermi level lies in a peak in the paramagnetic density of states, and the ferromagnetic phase is more stable. As first predicted by Schwarz, the magnetic moment is 2 \mu_B per Cr atom, with the Fermi level for minority spins lying in an insulating gap between oxygen p and chromium d states (""half-metallic"" behavior.) The A_1g Raman frequency is predicted to be 587 cm^{-1}. Drude plasma frequencies are of order 2eV, as seen experimentally by Chase. The measured resistivity is used to find the electron mean-free path l, which is only a few angstroms at 600K, but nevertheless, resistivity continues to rise as temperature increases. This puts CrO_2 into the category of ""bad metals"" in common with the high T_c superconductors, the high T metallic phase of VO_2, and the ferromagnet SrRuO_3. In common with both SrRuO_3 and Sr_2RuO_4, the measured specific heat \gamma is higher than band theory by a renormalization factor close to 4.",9608006v1 2013-01-13,A new lower limit for the bond breaking strains of defect-free carbon nanotubes: Tight binding MD simulation study,"The Order (N) Tight Binding Molecular Dynamics (TBMD) algorithms applied to simulate the tensile elongations of short (2-2.5 nm) armchair and zigzag Single Walled Carbon Nanotubes (SWCNTs) without bond breakings or defect formation. Simulations are repeated at high temperatures. We fix the lower limit of breaking strains to short SWCNTs without bond breaking or 5-7 defects formation. At room temperature, the simulated (4,4) SWCNT is able to carry the strain up to 130% of the relaxed tube length without bond breaking or 5-7 defects formation. This value is 127% for (11,0) SWCNT, 125% for (17,0) SWCNT, 123% for (10,10) SWCNT. In defect free, short nanotubes as the nanotube's radius increase the bond-breakings occur at lower strain values regardless of their chirality. This is true when we heat the tubes to higher temperatures. Bond breaking strain values, tensile strength, Young's modulus of the SWCNTs are obtained as functions of temperature. Defect free zigzag nanotubes exhibit higher tensile strength than armchaired ones. Young's modulus of defect free individual singlewall nanotubes is found to be in the range of 0.400 TPa within the elastic limit. At room temperature and experimentally realizable strain values, thinner tubes are more resistant to bond breaking and zigzag tubes over armchair ones. At high temperatures although the resistance to strain drops the same trend still holds. We observe a slight decrease of the tensile strength with increasing temperatures. The same trend is also observed in the Young's modulus. Results are important in determining a true breaking strains of SWCNTs.",1301.2786v1 2013-01-28,"Structural disorder, magnetism, and electrical and thermoelectric properties of pyrochlore Nd2Ru2O7","Polycrystalline Nd2Ru2O7 samples have been prepared and examined using a combination of structural, magnetic, and electrical and thermal transport studies. Analysis of synchrotron X-ray and neutron diffraction patterns suggests some site disorder on the A-site in the pyrochlore sublattice: Ru substitutes on the Nd-site up to 7.0(3)%, regardless of the different preparative conditions explored. Intrinsic magnetic and electrical transport properties have been measured. Ru 4d spins order antiferromagnetically at 143 K as seen both in susceptibility and specific heat, and there is a corresponding change in the electrical resistivity behaviour. A second antiferromagnetic ordering transition seen below 10 K is attributed to ordering of Nd 4f spins. Nd2Ru2O7 is an electrical insulator, and this behaviour is believed to be independent of the Ru-antisite disorder on the Nd site. The electrical properties of Nd2Ru2O7 are presented in the light of data published on all A2Ru2O7 pyrochlores, and we emphasize the special structural role that Bi3+ ions on the A-site play in driving metallic behaviour. High-temperature thermoelectric properties have also been measured. When considered in the context of known thermoelectric materials with useful figures-of-merit, it is clear that Nd2Ru2O7 has excessively high electrical resistivity which prevents it from being an effective thermoelectric. A method for screening candidate thermoelectrics is suggested.",1301.6661v1 2015-01-06,Coexistence of Electron-Glass Phase and Persistent Photoconductivity in GeSbTe Compounds,"It is demonstrated that persistent-photoconductivity (PPC), well-studied in lightly-doped semiconductors, is observable in GeSbTe compounds using infrared excitation at cryogenic temperatures. The low level of energy-flux necessary to induce an appreciable effect seems surprising given the high carrier-concentration n of these ternary alloys. On the other hand, their high density of carriers makes GeSbTe films favorable candidates for exhibiting intrinsic electron-glass effects with long relaxation times. These are indeed observed in GeSbTe thin-films that are Anderson-localized. In particular, a memory-dip is observed in samples with sheet resistances larger than app. 100 kOhms at T=4K with similar characteristics as in other systems that exhibit intrinsic electron-glass effects. Persistent-photoconductivity however is observable in GeSbTe films even for sheet resistances of the order of 1 kOhm, well below the range of disorder required for observing electron-glass effects. These two non-equilibrium phenomena, PPC and electron-glass, are shown to be of different nature in terms of other aspects as well. In particular, their relaxation dynamics is qualitatively different; the excess conductance dG/G associated with PPC decays with time as a stretched exponential whereas a logarithmic relaxation law characterizes dG(t) of all electron-glasses studied to date. Surprisingly, the magnitude of the memory-dip is enhanced when the system is in the PPC state. This counter-intuitive result may be related to the compositional disorder in these materials extending over mesoscopic scales. Evidence in support of this scenario is presented and discussed.",1501.01163v2 2018-11-05,Outstanding Radiation Resistance of Tungsten-based High Entropy Alloys,"A novel W-based refractory high entropy alloy with outstanding radiation resistance has been developed. The alloy was grown as thin films showing a bimodal grain size distribution in the nanocrystalline and ultrafine regimes and a unique 4 nm lamella-like structure revealed by atom probe tomography (APT). Transmission electron microscopy (TEM) and X-ray diffraction show an underlying body-centered cubic crystalline structure with certain black spots appearing after thermal annealing at elevated temperatures. Thorough analysis based on TEM and APT correlated the black spots with second phase particles rich in Cr and V. After both in situ and ex situ irradiation, these precipitates evolve to quasi-spherical particles with no sign of irradiation-created dislocation loops even after 8 dpa at either room temperature or 1073 K. Furthermore, nanomechanical testing shows a large hardness of 14 GPa in the as-deposited samples, with a slight increase after thermal annealing and almost negligible irradiation hardening. Theoretical modeling based on ab initio methodologies combined with Monte Carlo techniques predicts the formation of Cr and V rich second phase particles and points at equal mobilities of point defects as the origin of the exceptional radiation tolerance. The fact that these alloys are suitable for bulk production coupled with the exceptional radiation and mechanical properties makes them ideal structural materials for applications requiring extreme conditions.",1811.01915v1 2017-04-05,Cubic lead perovskite PbMoO3 with anomalous metallic behavior,"A previously unreported Pb-based perovskite PbMoO$_3$ is obtained by high-pressure and high-temperature synthesis. This material crystallizes in the $Pm\bar{3}m$ cubic structure at room temperature, making it distinct from typical Pb-based perovskite oxides with a structural distortion. PbMoO$_3$ exhibits a metallic behavior down to 0.1 K with an unusual $T$-sub linear dependence of the electrical resistivity. Moreover, a large specific heat is observed at low temperatures accompanied by a peak in $C_P/T^3$ around 10 K, in marked contrast to the isostructural metallic system SrMoO$_3$. These transport and thermal properties for PbMoO$_3$, taking into account anomalously large Pb atomic displacements detected through diffraction experiments, are attributed to a low-energy vibrational mode, associated with incoherent off-centering of lone pair Pb$^{2+}$ cations. We discuss the unusual behavior of the electrical resistivity in terms of a polaron-like conduction, mediated by the strong coupling between conduction electrons and optical phonons of the local low-energy vibrational mode.",1704.01270v1 2018-12-18,Hidden kagome-lattice picture and origin of high conductivity in delafossite PtCoO$_2$,"We study the electronic structure of delafossite PtCoO$_2$ to elucidate its extremely small resistivity and high mobility. The band exhibits steep dispersion near the Fermi level despite the fact that it is formed mainly by Pt $d$ orbitals that are typically localized. We propose a picture based on two hidden kagome-lattice-like electronic structure: one originating from Pt $s+p_x/p_y$ orbitals, and the other from Pt $d_{3z^2-r^2}+d_{xy}/d_{x^2-y^2}$ orbitals, each placed on the bonds of the triangular lattice. In particular, we find that the underlying Pt $s+p_x/p_y$ bands actually determine the steepness of the original dispersion, so that the large Fermi velocity can be attributed to the large width of the Pt $s+p_x/p_y$ band. More importantly, the kagome-like electronic structure gives rise to ""orbital-momentum locking"" on the Fermi surface, which reduces the electron scattering by impurities. We conclude that the combination of the large Fermi velocity and the orbital-momentum locking is likely to be the origin of the extremely small resistivity in PtCoO$_2$.",1812.07213v2 2019-10-29,Multi-frequency Shubnikov-de Haas oscillations in topological semimetal Pt$_2$HgSe$_3$,"Monolayer jacutingaite (Pt$_2$HgSe$_3$) has been recently identified as a candidate quantum spin Hall system with a 0.5 eV band gap, but no transport measurements have been performed so far on this material, neither in monolayer nor in the bulk. By using a dedicated high-pressure technique, we grow crystals enabling the exfoliation of 50-100 nm thick layers and the realization of devices for controlled transport experiments. Magnetoresistance measurements indicate that jacutingaite is a semimetal, exhibiting Shubnikov-de Haas (SdH) resistance oscillations with a multi-frequency spectrum. We adapt the Lifshitz-Kosevich formula to analyze quantitatively the SdH resistance oscillations in the presence of multiple frequencies, and find that the experimental observations are overall reproduced well by band structure ab-initio calculations for bulk jacutingaite. Together with the relatively high electron mobility extracted from the experiments ($\approx 2000$ cm$^2$/Vs, comparable to what is observed in WTe$_2$ crystals of the same thickness), our results indicate that monolayer jacutingaite should provide an excellent platform to investigate transport in 2D quantum spin Hall systems.",1910.13228v2 2020-10-11,Observation of Josephson-like tunneling junction characteristics and positive magnetoresistance in Oxygen deficient Nickelate films of $Nd_{0.8}Sr_{0.2}NiO_{3-δ}$,"Nickelate films have recently attracted broad attention due to the observation of superconductivity in the infinite layer phase of $Nd_{0.8}Sr_{0.2}NiO_2$ (obtained by reducing Sr doped $NdNiO_3$ films) and their similarity to the cuprates high temperature superconductors. Here we report on the observation of a new type of transport in oxygen poor $Nd_{0.8}Sr_{0.2}NiO_{3-\delta}$ films. At high temperatures, variable range hopping is observed while at low temperatures a novel tunneling behavior is found where Josephson-like tunneling junction characteristic with serial resistance is revealed. We attribute this phenomenon to coupling between superconductive (S) surfaces of the grains in our Oxygen poor films via the insulating (I) grain boundaries, which yields SIS junctions in series with the normal (N) resistance of the grains themselves. The similarity of the observed conductance spectra to tunneling junction characteristic with Josephson-like current is striking, and seems to support the existence of superconductivity in our samples.",2010.05277v2 2021-04-04,Mesoporous silica nanoparticles containing silver as novel antimycobacterial agents against Mycobacterium tuberculosis,"Tuberculosis remains today a major public health issue with a total of 9 million new cases and 2 million deaths annually. The lack of an effective vaccine and the increasing emergence of new strains of Mycobacterium tuberculosis (Mtb) highly resistant to antibiotics, anticipate a complicated scenario in the near future. The use of nanoparticles features as an alternative to antibiotics in tackling this problem due to their potential effectiveness in resistant bacterial strains. In this context, silver nanoparticles have demonstrated high bactericidal efficacy, although their use is limited by their relatively high toxicity, which calls for the design of nanocarriers that allow silver based nanoparticles to be safely delivered to the target cells or tissues. In this work mesoporous silica nanoparticles are used as carriers of silver based nanoparticles as antimycobacterial agent against Mtb. Two different synthetic approaches have been used to afford, on the one hand, a 2D hexagonal mesoporous silica nanosystem which contains silver bromide nanoparticles distributed all through the silica network and, on the other hand, a core@shell nanosystem with metallic silver nanoparticles as core and mesoporous silica shell in a radial mesoporous rearrangement. Both materials have demonstrated good antimycobacterial capacity in in vitro test using Mtb, being lower the minimum inhibitory concentration for the nanosystem which contains silver bromide. Therefore, the interaction of this material with the mycobacterial cell has been studied by cryo-electron microscopy, establishing a direct connection between the antimycobactericidal effect observed and the damage induced in the cell envelope.",2104.01649v1 2021-04-29,The dominance of non-electron-phonon charge carrier interaction in highly-compressed superhydrides,"The primary mechanism governing the emergence of near-room-temperature superconductivity in superhydrides is widely accepted to be the electron-phonon interaction. If so, the temperature dependent resistance, R(T), in these materials should obey the Bloch-Gr\""uneisen equation, where the power-law exponent, p, should be equal to the exact integer value of p=5. On the other hand, there is a well-established theoretical result that pure electron-magnon interaction should be manifested by p=3, and p=2 is the value for pure electron-electron interaction. Here we aimed to reveal the type of charge carrier interaction in the layered transition metal dichalcogenides PdTe2, high-entropy alloy (ScZrNb)0.65[RhPd]0.35, and highly-compressed elemental boron and superhydrides H3S, LaHx, PrH9 and BaH12 by fitting the temperature dependent resistance of these materials to the Bloch-Gr\""uneisen equation where the power-law exponent, p, is a free-fitting parameter. In the result, we showed that the high-entropy alloy (ScZrNb)0.65[RhPd]0.35 exhibited pure electron-phonon mediated superconductivity with p = 4.9. Unexpectedly we revealed that all studied superhydrides exhibit 1.8 < p < 3.2. This implies that it is unlikely that the electron-phonon interaction is the primary mechanism for the Cooper pairs formation in highly-compressed superhydrides and alternative pairing mechanisms, for instance, the electron-magnon, the electron-polaron, the electron-electron or other, should be considered as the origin for the emergence of near-room-temperature superconductivity in these compounds.",2104.14145v3 2021-09-30,Physical and Mechanical Properties of Cu-Fe System Functionally Graded and Multimaterial Structures after the DED,"This paper is devoted to experimental characterisation of linear thermal expansion coefficient (LTEC) and mechanical characteristics of the laser deposited Cu-Fe system multilayer functionally graded (FG) structures and binary Cu-Fe alloys, fabricated from the tin, aluminium, and chromium bronze with 89-99 wt.% of copper and stainless steel (SS) AISI 316L with 1:1 and 3:1 bronze-to-steel ratio. The best tensile mechanical strength of as-built parts is demonstrated by the aluminium bronze-stainless steel 1:1 alloy and reaches 876.4 MPa along with low elasticity modulus (11.2 GPa) and 1.684 1/K LTEC. Contrarily, the worst values of the mechanical characteristics are exhibited by parts created from the chromium bronze and SS, which failed at 294.0-463.3 MPa ultimate stress, showed the highest elasticity modulus (up to 42.4 GPa) and comparatively high average LTEC (up to 1.878 1/K). The aluminium bronze-stainless steel binary and FG alloys are discussed in the light of prospective application as the part of gradient materials, created by additive manufacturing (AM) technologies via the gradient path method and the alternating layers technique, with expected possibility of application in aerospace, nuclear, and electronic industry due to advantageous combination of the antifrictionality, heat conductivity, and oxidation resistance of the bronze, and the high mechanical strength, corrosion and creep resistance of the stainless steel.",2110.00103v1 2021-10-26,Temperature induced first order electronic topological transition in $β$-Ag$_2$Se,"$\beta$-Ag$_2$Se is a promising material for room temperature thermoelectric applications and magneto-resistive sensors. However, no attention was paid earlier to the hysteresis in the temperature dependence of resistivity ($\rho$($T$)). Here, we show that a broad hysteresis above 35 K is observed not only in $\rho$($T$), but also in other electronic properties such as Hall coefficient ($R_H$($T$)), Seebeck coefficient, thermal conductivity and ultraviolet photoelectron spectra (UPS). We also show that the hysteresis is not associated with a structural transition. The $\rho$($T$) and $R_H$($T$) show that $\beta$-Ag$_2$Se is semiconducting above 300 K, but metallicity is retained below 300 K. While electronic states are absent in the energy range from the Fermi level ($E_F$) to 0.4 eV below the $E_F$ at 300 K, a distinct Fermi edge is observed in the UPS at 15 K suggesting that the $\beta$-Ag$_2$Se undergoes an electronic topological transition from a high temperature semiconducting state to a low temperature metallic state. Our study reveals that a constant and moderately high thermoelectric figure of merit ($ZT$) in the range 300-395 K is observed due to the broad semiconductor to metal transition in $\beta$-Ag$_2$Se.",2110.13554v1 2021-11-11,Current-induced superconducting anisotropy of Sr$\mathsf{_2}$RuO$\mathsf{_4}$,"In the unconventional superconductor Sr$\mathsf{_2}$RuO$\mathsf{_4}$, unusual first-order superconducting transition has been observed in the low-temperature and high-field region, accompanied by a four-fold anisotropy of the in-plane upper critical magnetic field $H_{c2}$. The origin of such unusual $H_{c2}$ behavior should be closely linked to the debated superconducting symmetry of this oxide. Here, toward clarification of the unusual $H_{c2}$ behavior, we performed the resistivity measurements capable of switching in-plane current directions as well as precisely controlling the field directions. Our results reveal that resistive $H_{c2}$ under the in-plane current exhibits an additional two-fold anisotropy. By systematically analyzing $H_{c2}$ data taken under various current directions, we succeeded in separating the two-fold $H_{c2}$ component into the one originating from applied current and the other originating from certain imperfection in the sample. The former component, attributable to vortex flow effect, is weakened at low temperatures where $H_{c2}$ is substantially suppressed. The latter component is enhanced in the first order transition region, possibly reflecting a change in the nature of the superconducting state under high magnetic field.",2111.06097v1 2022-03-08,Electronic effects on the radiation damage in high-entropy alloys,"High-entropy alloys (HEAs) are exceptional candidates for radiation-resistant materials due to their complex local chemical environment and slow defect migration. Despite commonly overlooked, electronic effects on defects evolution in radiation environments also play a crucial role by dissipating excess energy through electron-phonon coupling and electronic heat conduction during cascade events. We present a systematic study on electronic properties in random-solid solutions (RSS) in four and five principal elements HEAs and their effect on defect formation, clustering, and recombination. Electronic properties, including electron-phonon coupling factor, the electronic specific heat, and the electronic thermal conductivity, are computed within first-principles calculations. Using the two-temperature molecular dynamics simulations, we show that the electron-phonon coupling factor and electronic specific heat play a critical role in Frenkel pairs formation. Specifically, the electron-phonon coupling factor quickly dissipates the kinetic energy during primary knock-on atom events via plasmon excitations and is subsequently dissipated via the free-electrons conduction. We show that these effects are more critical than the elastic distortion effects produced by the atomic mismatch. Of tremendous interest, we show that including lighter elements helps to increase the electron-phonon coupling factor, suggesting the possibility to improve radiation resistance in HEA through optimal composition.",2203.03779v2 2019-07-29,Linear-$T$ resistivity from low to high temperature: axion-dilaton theories,"The linear-$T$ resistivity is one of the hallmarks of various strange metals regardless of their microscopic details. Towards understanding this universal property, the holographic method or gauge/gravity duality has made much progress. Most holographic models have focused on the low temperature limit, where the linear-$T$ resistivity has been explained by the infrared geometry. We extend this analysis to high temperature and identify the conditions for a robust linear-$T$ resistivity up to high temperature. This extension is important because, in experiment, the linear-$T$ resistivity is observed in a large range of temperatures, up to room temperature. In the axion-dilaton theories we find that, to have a robust linear-$T$ resistivity, the strong momentum relaxation is a necessary condition, which agrees with the previous result for the Guber-Rocha model. However, it is not sufficient in the sense that, among large range of parameters giving a linear-$T$ resistivity in low temperature limit, only very limited parameters can support the linear-$T$ resistivity up to high temperature even in strong momentum relaxation. We also show that the incoherent term in the general holographic conductivity formula or the coupling between the dilaton and Maxwell term is responsible for a robust linear-$T$ resistivity up to high temperature.",1907.12168v3 2015-01-16,Phonon transmission across Mg2Si/Mg2Si1-xSnx interfaces: A first-principles-based atomistic Green's function study,"Phonon transmission across interfaces of dissimilar materials has been studied intensively in the recent years by using atomistic simulation tools owing to its importance in determining the effective thermal conductivity of nanostructured materials. Atomistic Green's function (AGF) method with interatomic force constants from the first-principles (FP) calculations has evolved to be a promising approach to study phonon transmission in many not well-studied material systems. However, the direct FP calculation for interatomic force constants becomes infeasible when the system involves atomic disorder. Mass approximation is usually used, but its validity has not been tested. In this paper, we employ the higher-order force constant model to extract harmonic force constants from the FP calculations, which originates from the virtual crystal approximation but considers the local force-field difference. As a feasibility demonstration of the proposed method that integrates higher-order force constant model from the FP calculations with the AGF, we study the phonon transmission in the Mg2Si/Mg2Si1-xSnx systems. When integrated with the AGF, the widely-used mass approximation is found to overpredict phonon transmission across Mg2Si/Mg2Sn interface. The difference can be attributed to the absence of local strain field-induced scattering in the mass approximation, which makes the high-frequency phonons less scattered. The frequency-dependent phonon transmission across an interface between a crystal and an alloy, which often appears in high efficiency ""nanoparticle in alloy"" thermoelectric materials, is studied. The interfacial thermal resistance across Mg2Si/Mg2Si1-xSnx interface is found to be weakly dependent on the composition of Sn when the composition x is less than 40%, but increases rapidly when it is larger than 40% due to the transition of high-frequency phonon DOS in Mg2Si1-xSnx alloys.",1501.04084v1 2020-06-19,Dionysian Hard Sphere Packings are Mechanically Stable at Vanishingly Low Densities,"High strength-to-weight ratio materials can be constructed by either maximizing strength or minimizing weight. Tensegrity structures and aerogels take very different paths to achieving high strength-to-weight ratios but both rely on internal tensile forces. In the absence of tensile forces, removing material eventually destabilizes a structure. Attempts to maximize the strength-to-weight ratio with purely repulsive spheres have proceeded by removing spheres from already stable crystalline structures. This results in a modestly low density and a strength-to-weight ratio much worse than can be achieved with tensile materials. Here, we demonstrate the existence of a packing of hard spheres that has asymptotically zero density and yet maintains finite strength, thus achieving an unbounded strength-to-weight ratio. This construction, which we term Dionysian, is the diametric opposite to the Apollonian sphere packing which completely and stably fills space. We create tools to evaluate the stability and strength of compressive sphere packings. Using these we find that our structures have asymptotically finite bulk and shear moduli and are linearly resistant to every applied deformation, both internal and external. By demonstrating that there is no lower bound on the density of stable structures, this work allows for the construction of arbitrarily lightweight high-strength materials.",2006.11415v3 2020-06-30,Electrothermal Transport Induced Material Re Configuration and Performance Degradation of CVD Grown Monolayer MoS2 Transistors,"We report, for CVD-grown monolayer MoS2, the very first results on temporal degradation of material and device performance under electrical stress. Both low and high field regimes of operation are explored at different temperatures, gate bias and stress cycles. During low field operation, current is found to saturate after hundreds of seconds of operation with the current decay time constant being a function of temperature and stress cycle. Current saturation after several seconds during low field operation occurs when a thermal equilibrium is established. However, high field operation, especially at low temperature, leads to impact ionization assisted material and device degradation. It is found that high field operation at low temperature results in amorphization of the channel and is verified by device and Kelvin Probe Force Microscopy (KPFM) analyses. In general, a prolonged room temperature operation of CVD-grown MoS2 transistors lead to degraded gate control, higher OFF state current and negative shift in threshold voltage (VT). This is further verified, through micro-Raman and Photoluminescence spectroscopy, which suggest that a steady state DC electrical stress leads to the formation of localized low resistance regions in the channel and a subsequent loss of transistor characteristics. Our findings unveil unique mechanism by which CVD MoS2 undergoes material degradation under electrical stress and subsequent breakdown of transistor behavior. Such an understanding of material and device reliability helps in determining the safe operating regime from device as well as circuit perspective.",2006.16952v1 2020-08-12,High Rate Hybrid MnO2@CNT Fabric Anode for Li-Ion Batteries: Properties and Lithium Storage Mechanism by In-Situ Synchrotron X-Ray Scattering,"High-performance anodes for rechargeable Li-ion battery are produced by nanostructuring of the transition metal oxides on a conductive support. Here, we demonstrate a hybrid material of MnO2 directly grown onto fabrics of carbon nanotube fibres, which exhibits notable specific capacity over 1100 and 500 mAh/g at a discharge current density of 25 mA/g and 5 A/g, respectively, with coulombic efficiency of 97.5 %. Combined with 97 % capacity retention after 1500 cycles at a current density of 5 A/g, both capacity and stability are significantly above literature data. Detailed investigations involving electrochemical and in situ synchrotron X-ray scattering study reveal that during galvanostatic cycling, MnO2 undergoes an irreversible phase transition to LiMnO2, which stores lithium through an intercalation process, followed by conversion mechanism and pseudocapacitive processes. This mechanism is further confirmed by Raman spectroscopy and X-ray photoelectron spectroscopy. The fraction of pseudocapacitive charge storage ranges from 27% to 83%, for current densities from 25 mA/g to 5 A/g. Firm attachment of the active material to the built-in current collector makes the electrodes flexible and mechanically robust, and ensures that the low charge transfer resistance and the high electrode surface area remain after irreversible phase transition of the active material and extensive cycling.",2008.05169v1 2021-12-01,Unraveling diffusion kinetics of honeycomb structured Na$_2$Ni$_2$TeO$_6$ as a high-potential and stable electrode for sodium-ion batteries,"In search of the potential cathode materials for sodium-ion batteries and to understand the diffusion kinetics, we report the detailed analysis of electrochemical investigation of honeycomb structured Na$_{2}$Ni$_{2}$TeO$_{6}$ material using cyclic voltammetry (CV), electrochemical impedance spectroscopy (EIS), galvanostatic charge-discharge (GCD) and galvanostatic intermittent titration technique (GITT). We found the discharge capacities of 82 and 77 mAhg$^{-1}$ at 0.05~C and 0.1~C current rates, respectively, and the mid-working potential of $\approx$3.9~V at 1~C and high capacity retention of 80\% after 500 cycles at 0.5~C as well as excellent rate capability. The analysis of CV data at different scan rates reveals the pseudo-capacitive mechanism of sodium-ion storage. Interestingly, the {\it in-situ} EIS measurements show a systematic change in the charge-transfer resistance at different charge/discharge stages as well as after different number of cycles. The diffusion coefficient extracted using CV, EIS and GITT lies mainly in the range of 10$^{-10}$ to 10$^{-12}$ cm$^{2}$s$^{-1}$ and the de-insertion/insertion of Na$^+$-ion concentration during electrochemical cycling is consistent with the ratio of Ni$^{3+}$/Ni$^{2+}$ valence state determined by photoemission study. Moreover, the post-cyclic results of retrieved active material show very stable structure and morphology even after various charge-discharge cycles. Our detailed electrochemical investigation and diffusion kinetics studies establish the material as a high working potential and long life electrode for sodium-ion batteries.",2112.00536v1 2000-04-19,Role of in-plane dissipation in dynamics of Josephson lattice in high-temperature superconductors,"We calculate the flux-flow resistivity of the Josephson vortex lattice in a layered superconductor taking into account both the inter-plane and in-plane dissipation channels. We consider the limiting cases of small fields (isolated vortices) and high fields (overlapping vortices). In the case of the dominating in-plane dissipation, typical for high-temperature superconductors, the field dependence of flux-flow resistivity is characterized by {\it three} distinct regions. As usual, at low fields the flux-flow resistivity grows linearly with field. When the Josephson vortices start to overlap the flux-flow resistivity crosses over to the regime of {\it quadratic} field dependence. Finally, at very high fields the flux-flow resistivity saturates at the c-axis quasiparticle resistivity. The intermediate quadratic regime indicates dominant role of the in-plane dissipation mechanism. Shape of the field dependence of the flux-flow resistivity can be used to extract both components of the quasiparticle",0004337v2 2014-11-24,Spatial heterogeneity in drug concentrations can facilitate the emergence of resistance to cancer therapy,"Acquired resistance is one of the major barriers to successful cancer therapy. The development of resistance is commonly attributed to genetic heterogeneity. However, heterogeneity of drug penetration of the tumor microenvironment both on the microscopic level within solid tumors as well as on the macroscopic level across metastases may also contribute to acquired drug resistance. Here we use mathematical models to investigate the effect of drug heterogeneity on the probability of escape from treatment and time to resistance. Specifically we address scenarios with sufficiently efficient therapies that suppress growth of all preexisting genetic variants in the compartment with highest drug concentration. To study the joint effect of drug heterogeneity, growth rate, and evolution of resistance we analyze a multitype stochastic branching process describing growth of cancer cells in two compartments with different drug concentration and limited migration between compartments. We show that resistance is more likely to arise first in the low drug compartment and from there populate the high drug compartment. Moreover, we show that only below a threshold rate of cell migration does spatial heterogeneity accelerate resistance evolution, otherwise deterring drug resistance with excessively high migration rates. Our results provide new insights into understanding why cancers tend to quickly become resistant, and that cell migration and the presence of sanctuary sites with little drug exposure are essential to this end.",1411.6684v1 2018-10-23,Relativistic resistive magnetohydrodynamic reconnection and plasmoid formation in merging flux tubes,"We apply the general relativistic resistive magnetohydrodynamics code {\tt BHAC} to perform a 2D study of the formation and evolution of a reconnection layer in between two merging magnetic flux tubes in Minkowski spacetime. Small-scale effects in the regime of low resistivity most relevant for dilute astrophysical plasmas are resolved with very high accuracy due to the extreme resolutions obtained with adaptive mesh refinement. Numerical convergence in the highly nonlinear plasmoid-dominated regime is confirmed for a sweep of resolutions. We employ both uniform resistivity and non-uniform resistivity based on the local, instantaneous current density. For uniform resistivity we find Sweet-Parker reconnection, from $\eta = 10^{-2}$ down to $\eta = 10^{-4}$, for a reference case of magnetisation $\sigma = 3.33$ and plasma-$\beta = 0.1$. {For uniform resistivity $\eta=5\times10^{-5}$ the tearing mode is recovered, resulting in the formation of secondary plasmoids. The plasmoid instability enhances the reconnection rate to $v_{\rm rec} \sim 0.03c$ compared to $v_{\rm rec} \sim 0.01c$ for $\eta=10^{-4}$.} For non-uniform resistivity with a base level $\eta_0 = 10^{-4}$ and an enhanced current-dependent resistivity in the current sheet, we find an increased reconnection rate of $v_{\rm rec} \sim 0.1c$. The influence of the magnetisation $\sigma$ and the plasma-$\beta$ is analysed for cases with uniform resistivity $\eta=5\times10^{-5}$ and $\eta=10^{-4}$ in a range $0.5 \leq \sigma \leq 10$ and $0.01 \leq \beta \leq 1$ in regimes that are applicable for black hole accretion disks and jets. The plasmoid instability is triggered for Lundquist numbers larger than a critical value of $S_{\rm c} \approx 8000$.",1810.10116v2 2023-11-06,Quantification of spin-charge interconversion in highly resistive sputtered Bi$_x$Se$_{1-x}$ with non-local spin valves,"The development of spin-orbitronic devices, such as magneto-electric spin-orbit logic devices, calls for materials with a high resistivity and a high spin-charge interconversion efficiency. One of the most promising candidates in this regard is sputtered Bi$_x$Se$_{1-x}$. Although there are several techniques to quantify spin-charge interconversion, to date reported values for sputtered Bi$_x$Se$_{1-x}$ have often been overestimated due to spurious effects related to local currents combined with a lack of understanding of the effect of the interfaces and the use of approximations for unknown parameters, such as the spin diffusion length. In the present study, non-local spin valves are used to inject pure spin currents into Bi$_x$Se$_{1-x}$, allowing us to directly obtain its spin diffusion length as well as its spin Hall angle, from 10 K up to 300 K. These values, which are more accurate than those previously reported in sputtered Bi$_x$Se$_{1-x}$, evidence that the efficiency of this material is not exceptional. Indeed, the figure of merit for spin-charge interconversion, given by the product of these two parameters, is slightly under 1 nm. Our work demonstrates the importance of considering all material parameters and interfaces when quantifying the spin transport properties of materials with strong spin-orbit coupling.",2311.03598v1 2015-02-10,Dichotomy between the hole and electrons behavior in the multiband FeSe probed by ultra high magnetic fields,"Magnetoresistivity \r{ho}xx and Hall resistivity \r{ho}xy in ultra high magnetic fields up to 88T are measured down to 0.15K to clarify the multiband electronic structure in high-quality single crystals of superconducting FeSe. At low temperatures and high fields we observe quantum oscillations in both resistivity and Hall effect, confirming the multiband Fermi surface with small volumes. We propose a novel and independent approach to identify the sign of corresponding cyclotron orbit in a compensated metal from magnetotransport measurements. The observed significant differences in the relative amplitudes of the quantum oscillations between the \r{ho}xx and \r{ho}xy components, together with the positive sign of the high-field \r{ho}xy , reveal that the largest pocket should correspond to the hole band. The low-field magnetotransport data in the normal state suggest that, in addition to one hole and one almost compensated electron bands, the orthorhombic phase of FeSe exhibits an additional tiny electron pocket with a high mobility.",1502.02922v1 2023-10-31,Unlocking ultrastrong high-temperature ceramics: Beyond Equimolar Compositions in High Entropy Nitrides,"Traditionally, increasing compositional complexity and chemical diversity of high entropy alloy ceramics whilst maintaining a stable single-phase solid solution has been a primary design strategy for the development of new ceramics. However, only a handful have shown properties that justify the increased alloying content. Here, we unveil a groundbreaking strategy based on deviation from conventional equimolar composition towards non-equimolar composition space, enabling tuning the metastability level of the supersaturated single-phase solid solution. By employing high-temperature micromechanical testing of refractory metal-based high entropy nitrides, we found that the activation of an additional strengthening mechanism upon metastable phase decomposition propels the yield strength of a non-equimolar nitride at 1000 C to a staggering 6.9 GPa, that is 40 % higher than the most robust equimolar nitride. We show that the inherent instability triggers the decomposition of the solid solution with non-equimolar composition at high temperatures, inducing strengthening due to the coherency stress of a spinodally modulated structure, combined with the lattice resistance of the product solid solution phase. In stark contrast, the strength of equimolar systems, boasting diverse chemical compositions, declines as a function of temperature due to the weakening of the lattice resistance and the absence of other strengthening mechanisms.",2310.20441v2 2010-09-21,Large yield production of high mobility freely suspended graphene electronic devices on a PMGI based organic polymer,"The recent observation of fractional quantum Hall effect in high mobility suspended graphene devices introduced a new direction in graphene physics, the field of electron-electron interaction dynamics. However, the technique used currently for the fabrication of such high mobility devices has several drawbacks. The most important is that the contact materials available for electronic devices are limited to only a few metals (Au, Pd, Pt, Cr and Nb) since only those are not attacked by the reactive acid (BHF) etching fabrication step. Here we show a new technique which leads to mechanically stable suspended high mobility graphene devices which is compatible with almost any type of contact material. The graphene devices prepared on a polydimethylglutarimide based organic resist show mobilities as high as 600.000 cm^2/Vs at an electron carrier density n = 5.0 10^9 cm^-2 at 77K. This technique paves the way towards complex suspended graphene based spintronic, superconducting and other types of devices.",1009.4213v2 2024-02-04,"High temperature internal friction in a Ti-46Al-1Mo-0.2Si intermetallic, comparison with creep behaviour","Advanced g-TiAl based intermetallics Mo-bearing have been developed to obtain the fine-grained microstructure required for superplastic deformation to be used during further processing. In the present work we have studied an alloy of Ti-46Al-1Mo-0.2Si (at%) with two different microstructures, as-cast material with a coarse grain size above 300 mm, and the hot extruded material exhibiting a grain size smaller than 20 mm. We have used a mechanical spectrometer especially developed for high temperature internal friction measurements to study the defect mobility processes taking place at high temperature. The internal friction spectra at different frequencies has been studied and analyzed up to 1360 K in order to characterize the relaxation processes appearing in this temperature range. A relaxation peak, with a maximum in between 900 K and 1080 K, depending on the oscillating frequency, has been attributed to Ti-atoms diffusion by the stress-induced reorientation of Al-VTi-Al elastic dipoles. The high temperature background in both microstructural states, as-cast and extruded, has been analyzed, measuring the apparent activation parameters, in particular the apparent energies of Ecast(IF) 4.4 +- 0.05 eV and Eext(IF) 4.75 +- 0.05 eV respectively. These results have been compared to those obtained on the same materials by creep deformation. We may conclude that the activation parameters obtained by internal friction analysis, are consistent with the ones measured by creep. Furthermore, the analysis of the high temperature background allows establish the difference on creep resistance for both microstructural states",2402.03389v1 1997-03-03,Evidence for Kondo Effect in Au80Co20 Ribbons,"A minimum in resistivity as a function of temperature for an as-quenched Au80Co20 ribbon prepared by melt-spinning using a wheel surface speed of 20 m s^{-1} is found at 25 K. No resistivity minimum is found for an as-quenched ribbon using a wheel surface speed of 60 m s^{-1}, however, upon heat treatment of this ribbon a resistivity minimum is recovered. The temperature of the minimum decreases with increasing total time of heat treatment. These observations are interpretted as evidence for the microstructural control of the Kondo effect typically found in dilute magnetic alloys in a giant magnetoresistance granular material.",9703030v1 2006-05-18,Intrinsic inhomogeneities and effects of resistive switching in doped manganites,"The effect of resistive switching in doped manganites being in the ferromagnetic state has been studied using resistive and magneto-optic methods. The visualization of magnetic structure of La0.75Sr0.25MnO3-x single crystals, and its transformation under electric current proposed local superheating of the material above the Curie temperature, which was supported by numerical calculation. The obtained results suggest a significant role of micrometer-scale inhomogeneity of manganites in phase separation, magnetic and transport properties of the material.",0605457v1 2008-04-29,Resistivity reduction of boron-doped multi-walled carbon nanotubes synthesized from a methanol solution containing a boric acid,"Boron-doped multi-walled carbon nanotubes (MWNTs) were synthesized using a methanol solution of boric acid as a source material. Accurate measurements of the electrical resistivity of an individual boron-doped MWNT was performed with a four-point contact, which was fabricated using an electron beam lithography technique. The doped boron provides conduction carriers, which reduces the resistivity of the MWNT.",0804.4514v1 2018-12-20,"Layer-by-layer resistive switching: multi-state functionality due to electric-field-induced healing of ""dead"" layers","Materials exhibiting reversible resistive switching in electrical fields are highly demanded for functional elements in oxide electronics. In particular, multilevel switching effects allow for advanced applications like neuromorphic circuits. Here we report on a structurally driven switching mechanism involving the so-called `dead layers' of perovskite manganite surfaces. Forming a tunnel barrier whose thickness can be changed in monolayer steps by electrical fields, the switching effect exhibits well-defined and robust resistive states.",1812.08563v1 2019-10-29,Improvement in corrosion resistance and biocompatibility of AZ31 magnesium alloy by NH+2 ions,"Magnesium alloys have been considered to be favorable biodegradable metallic materials used in orthopedic and cardiovascular applications. We introduce NH+2 to the AZ31 Mg alloy surface by ion implantation at the energy of 50 KeV with doses ranging from 1e16 ions/cm2 to 1e17 ions/cm2 to improve its corrosion resistance and biocompatibility. Surface morphology, mechanical properties, corrosion behavior and biocompatibility are studied in the experiments. The analysis confirms that the modified surface with smoothness and hydrophobicity significantly improves the corrosion resistance and biocompatibility while maintaining the mechanical property of the alloy.",1910.13265v1 2020-01-08,UV-laser modification and selective ion-beam etching of amorphous vanadium pentoxide thin films,"We present the results on excimer laser modification and patterning of amorphous vanadium pentoxide films. Wet positive resist-type and Ar ion-beam negative resist-type etching techniques were employed to develop UV-modified films. V2O5 films were found to possess sufficient resistivity compared to standard electronic materials thus to be promising masks for sub-micron lithog-raphy",2001.03054v1 2006-06-20,Phase study of oscillatory resistances in high mobility GaAs/AlGaAs devices: Indications of a new class of integral quantum Hall effect,"An experimental study of the high mobility GaAs/AlGaAs system at large-$\nu$ indicates several distinct phase relations between the oscillatory diagonal- and Hall- resistances, and suggests a new class of integral quantum Hall effect, which is characterized by ""anti-phase"" Hall- and diagonal- resistance oscillations.",0606517v1 2017-09-15,Spontaneous surface reserve formation in wicked membranes bestow extreme stretchability,"Soft stretchable materials are key for arising technologies such as stretchable electronics or batteries, smart textiles, biomedical devices, tissue engineering and soft robotics. Recent attempts to design such materials, via e.g. micro-patterning of wavy fibres on soft substrates, polymer engineering at the molecular level or even kirigami techniques, provide appealing prospects but suffer drawbacks impacting the material viability: complexity of manufacturing, fatigue or failure upon cycling, restricted range of materials or biological incompatibility. Here, we report a universal strategy to design highly stretchable, self-assembling and fatigue-resistant synthetic fabrics. Our approach finds its inspiration in the mechanics of living animal cells that routinely encounter and cope with extreme deformations, e.g. with the engulfment of large intruders by macrophages, squeezing and stretching of immune cells in tiny capillaries or shrinking/swelling of neurons upon osmotic stimuli. All these large instant deformations are actually mediated and buffered by membrane reserves available in the form of microvilli, membrane folds or endomembrane that can be recruited on demand. We synthetically mimicked this behavior by creating nanofibrous liquid-infused tissues spontaneously forming surface reserves whose unfolding fuels any imposed shape change. Our process, relying only on geometry, elasticity and capillarity, allows to endow virtually any material with high stretchability and reversibility, making it straightforward to implement additional mechanical, electrical or chemical functions. We illustrate this with proof-of-concept activable capillary muscles, adaptable slippery liquid infused porous surfaces and stretchable basic printed electronic circuits.",1709.05228v1 2018-02-26,Trilayer TMDC Heterostructures for MOSFETs and Nanobiosensors,"Two dimensional materials such as Transition Metal Dichalcogenides (TMDC) and their bi-layer/tri-layer heterostructures have become the focus of intense research and investigation in recent years due to their promising applications in electronics and optoelectronics. In this work, we have explored device level performance of trilayer TMDC heterostructure (MoS2/MX2/MoS2; M=Mo or, W and X=S or, Se) Metal Oxide Semiconductor Field Effect Transistors (MOSFETs) in the quantum ballistic regime. Our simulation shows that device 'on' current can be improved by inserting a WS2 monolayer between two MoS2 monolayers. Application of biaxial tensile strain reveals a reduction in drain current which can be attributed to the lowering of carrier effective mass with increased tensile strain. In addition, it is found that gate underlap geometry improves electrostatic device performance by improving sub-threshold swing. However, increase in channel resistance reduces drain current. Besides exploring the prospect of these materials in device performance, novel trilayer TMDC heterostructure double gate Field Effect Transistors (FETs) are proposed for sensing Nano biomolecules as well as for pH sensing. Bottom gate operation ensures these FETs operating beyond Nernst limit of 59 mV/pH. Simulation results found in this work reveal that scaling of bottom gate oxide results in better sensitivity while top oxide scaling exhibits an opposite trend. It is also found that, for identical operating conditions, proposed TMDC FET pH sensors show super-Nernst sensitivity indicating these materials as potential candidates in implementing such sensor. Besides pH sensing, all these materials show high sensitivity in the sub-threshold region as a channel material in nanobiosensor while MoS2/WS2/MoS2 FET shows the least sensitivity among them.",1802.09141v1 2018-06-07,Plasmonics in Argentene,"Two-dimensional materials exhibit a fascinating range of electronic and photonic properties vital for nanophotonics, quantum optics and emerging quantum information technologies. Merging concepts from the fields of ab initio materials science and nanophotonics, there is now an opportunity to engineer new photonic materials whose optical, transport, and scattering properties are tailored to attain thermodynamic and quantum limits. Here, we present first-principles calculations predicting that Argentene, a single-crystalline hexagonal close-packed monolayer of Ag, can dramatically surpass the optical properties and electrical conductivity of conventional plasmonic materials. In the low-frequency limit, we show that the scattering rate and resistivity reduce by a factor of three compared to the bulk three-dimensional metal. Most importantly, the low scattering rate extends to optical frequencies in sharp contrast to e.g. graphene, whose scattering rate increase drastically in the near-infrared range due to optical-phonon scattering. Combined with an intrinsically high carrier density, this facilitates highly-confined surface plasmons extending to visible frequencies. We evaluate Argentene across three distinct figures of merit, spanning the spectrum of typical plasmonic applications; in each, Argentene outperforms the state-of-the-art. This unique combination of properties will make Argentene a valuable addition to the two-dimensional heterostructure toolkit for quantum electronic and photonic technologies.",1806.02672v1 2023-03-22,Enhanced functional reversibility in lead-free ferroelectric material over long cycle pyroelectric energy conversion,"The ferroelectric material usually exhibits temperature dependent spontaneous polarization, known as pyroelectricity, which can be used to directly convert thermal energy to electricity from ambient low-grade waste heat. When utilizing the structural phase transformations of the material, the conversion capability can be magnified, consequently the device performance can be strongly boosted by orders of magnitude. However, common ferroelectric oxides suffer the mechanical fatigue and functional degradation over cyclic phase transformations, hindering widespread applications of the energy conversion device. In this paper, we investigate the mechanical and functional reversibility of the material by lattice tuning and grain coarsening. We discover the lead-free compound Ba(Ce$_{0.005}$Zr$_{0.005}$)Ti$_{0.99}$O3-0.10(Ba$_{0.7}$Ca$_{0.3}$)TiO$_3$ (BCZT-0.10BCT) satisfying the compatibility condition among all present phases by its lattice parameters, making the phase transformations highly reversible. We demonstrated that the energy conversion device with the equiaxial coarse grains exhibits exceptional fatigue-resistance, with stable pyroelectric current output at 4$\mu$A/cm$^2$ over 3,000 energy conversion cycles. Our work opens a new way to fabricate high-performance material that advances the pyroelectric energy conversion for practical application in engineering.",2303.12583v1 2023-04-28,Computational study of III-V direct-gap semiconductors for thermoradiative cell applications,"We investigate the performance of thermoradiative (TR) cells using the III-V group of semiconductors, which include GaAs, GaSb, InAs, and InP, with the aim of determining their efficiency and finding the best TR cell materials among the III-V group. The TR cells generate electricity from thermal radiation, and their efficiency is influenced by several factors such as the bandgap, temperature difference, and absorption spectrum. To create a realistic model, we incorporate sub-bandgap and heat losses in our calculations and utilize density-functional theory to determine the energy gap and optical properties of each material. Our findings suggest that the effect of absorptivity on the material, especially when the sub-bandgap and heat losses are considered, can decrease the efficiency of TR cells. However, careful treatment of the absorptivity indicates that not all materials have the same trend of decrease in the TR cell efficiency when taking the loss mechanisms into account. We observe that GaSb exhibits the highest power density, while InP demonstrates the lowest one. Moreover, GaAs and InP exhibit relatively high efficiency without the sub-bandgap and heat losses, whereas InAs display lower efficiency without considering the losses, yet exhibit higher resistance to sub-bandgap and heat losses compared to the other materials, thus effectively becoming the best TR cell material in the III-V group of semiconductors.",2304.14917v1 2005-12-21,"Poly-MTO, {(CH_3)_{0.92} Re O_3}_\infty, a Conducting Two-Dimensional Organometallic Oxide","Polymeric methyltrioxorhenium, {(CH_{3})_{0.92}ReO_{3}}_{\infty} (poly-MTO), is the first member of a new class of organometallic hybrids which adopts the structural pattern and physical properties of classical perovskites in two dimensions (2D). We demonstrate how the electronic structure of poly-MTO can be tailored by intercalation of organic donor molecules, such as tetrathiafulvalene (TTF) or bis-(ethylendithio)-tetrathiafulvalene (BEDT-TTF), and by the inorganic acceptor SbF$_3$. Integration of donor molecules leads to a more insulating behavior of poly-MTO, whereas SbF$_3$ insertion does not cause any significant change in the resistivity. The resistivity data of pure poly-MTO is remarkably well described by a two-dimensional electron system. Below 38 K an unusual resistivity behavior, similar to that found in doped cuprates, is observed: The resistivity initially increases approximately as $\rho \sim$ ln$(1/T$) before it changes into a $\sqrt{T}$ dependence below 2 K. As an explanation we suggest a crossover from purely two-dimensional charge-carrier diffusion within the \{ReO$_2$\}$_{\infty}$ planes at high temperatures to three-dimensional diffusion at low temperatures in a disorder-enhanced electron-electron interaction scenario (Altshuler-Aronov correction). Furthermore, a linear positive magnetoresistance was found in the insulating regime, which is caused by spatial localization of itinerant electrons at some of the Re atoms, which formally adopt a $5d^1$ electronic configuration. X-ray diffraction, IR- and ESR-studies, temperature dependent magnetization and specific heat measurements in various magnetic fields suggest that the electronic structure of poly-MTO can safely be approximated by a purely 2D conductor.",0512544v1 2017-10-10,Clustered vacancies in ZnO: Chemical aspects and consequences on physical properties,"Chemical nature of point defects, their segregation, cluster or complex formation in ZnO is an important area of investigation. In this report, 1.2 MeV Ar ion beam is used to incorporate defects in granular ZnO. Evolution of defective state with irradiation fluence 1 x 10^14 and 1 x 10^16 ions/cm2 has been monitored using XPS, PL and Raman spectroscopic study. XPS study shows presence of oxygen vacancies (VO) in the Ar ion irradiated ZnO. Zn(LMM) Auger spectra clearly identifies transition involving metallic zinc in the irradiated samples. Intense PL emission from IZn related shallow donor bound excitons (DBX) is visible in the 10 K spectra for all samples. Although overall PL is largely reduced with irradiation disorder, DBX intensity is increased for the highest fluence irradiated sample. Raman study indicates damage in both zinc and oxygen sub-lattice by energetic ion beam. Representative Raman modes from defect complexes involving VO, IZn and IO are visible after irradiation with intermediate fluence. Further increase of fluence shows, to some extent, a homogenization of disorder. Huge reduction of resistance is also noted for this sample. Certainly, high irradiation fluence induces a qualitative modification of the conventional (and highly resistive) grain boundary (GB) structure of granular ZnO. Low resistive path, involving IZn related shallow donors, across the GB can be presumed to explain resistance reduction. Open volumes (VZn and VO) agglomerate more and more with increasing irradiation fluence and finally get transformed to voids. Results as a whole have been elucidated with a model which emphasizes possible evolution of new defect microstructure that is distinctively different from the GB related disorder. Based on the model, qualitative explanations of commonly observed radiation hardness, colouration and ferromagnetism in disordered ZnO have been put forward.",1710.03696v1 2021-09-23,Zero Magnetic Field Plateau Phase Transition in Higher Chern Number Quantum Anomalous Hall Insulators,"The plateau-to-plateau transition in quantum Hall effect under high magnetic fields is a celebrated quantum phase transition between two topological states through either sweeping the magnetic field or tuning the carrier density. The recent realization of the quantum anomalous Hall (QAH) insulators with tunable Chern numbers introduces the channel degree of freedom to the dissipation-free chiral edge transport and makes the study of the quantum phase transition between two topological states under zero magnetic field possible. Here, we synthesized the magnetic topological insulator (TI)/TI penta-layer heterostructures with different Cr doping concentrations in the middle magnetic TI layers using molecular beam epitaxy (MBE). By performing transport measurements, we found a zero magnetic field quantum phase transition between the C = 1 and C = 2 QAH states. In tuning the transition, the Hall resistance monotonically decreases from h/e2 to h/2e2, concurrently, the longitudinal resistance exhibits a maximum at the critical point. Our results show that the ratio between the Hall resistance and the longitudinal resistance is greater than 1 at the critical point, which indicates that the original chiral edge channel from the C = 1 QAH state coexists with the dissipative bulk conduction channels. Subsequently, these bulk conduction channels appear to self-organize and form the second chiral edge channel in completing the plateau phase transition. Our study will motivate further investigations of this novel Chern number change-induced quantum phase transition and advance the development of the QAH chiral edge current-based electronic and spintronic devices.",2109.11382v1 2023-07-15,Planar Hall effect and Anisotropic Magnetoresistance in Thin Films of Chiral Antiferromagnet Mn3Sn,"Antiferromagnetic Weyl semimetals with spin chirality offer excellent platforms to address the Berry phase physics, which manifests prominently in several of their electro-optical and electro-magnetic responses including as a large anomalous Hall effect (AHE) and spin Hall conductivity. Here, we report measurements of magneto-transport in c-axis textured Mn3Sn thin films grown on the [111] plane of single crystal MgO. At room temperature, these films display a weak uncompensated magnetic moment of \approx 0.12 \micro_{B}/f.u. in the basal plane and a longitudinal resistivity (\rho_{xx}) close to \approx 3.8 \micro\Omega.m. A residual resistivity ration (\rho_{xx} (300 K)/\rho_{xx} (2 K)) of \approx 3.92 further indicates the high quality of the films. While at 300 K a weak AHE together with field-linear Hall resistivity (\rho_{xy}) is observed in magnetic fields (H) applied perpendicular to the Kagome planes, the temperature (T) dependence of \rho_{xy} shows prominent signatures of three magnetic phases in the temperature regime of 2 to 300 K. The \rho_{xy} also derives a non-trivial topological contribution (\r{ho}THE \approx 1n\Omega.m) in the spin glass phase which appears at T \geq 100 K. Our measurements of anisotropic magnetoresistance (AMR) and planar Hall effect (PHE) over a wide H-T phase space reveal the hitherto unseen effects in the three magnetic phases of Mn3Sn. While the AMR and PHE are negative in the inverse triangular spin phase (250 K \geq T \geq TN), the helical phase (100 \geq T \geq 250 K) is devoid of anisotropic in-plane resistivity, and the spin glass phase shows a sign reversal of AMR with the increasing magnetic field. The origin of this sign change in AMR/PHE is attributed to the emergence of topologically protected spin textures like skyrmions where the fictitious effective magnetic field is estimated to be \approx 4.4 tesla.",2307.07795v1 2024-02-27,"Field, frequency and temperature dependence of the surface resistance of nitrogen diffused niobium superconducting radio frequency cavities","We report the RF performance of several single-cell superconducting radio-frequency cavities subjected to low temperature heat treatment in nitrogen environment. The cavities were treated at temperature 120 - 165 $^{\circ}$C for an extended period of time (24 - 48 hours) either in high vacuum or in a low partial pressure of ultra-pure nitrogen. The improvement in $Q_0$ with a Q-rise was observed when nitrogen gas was injected at $\sim$300 $^{\circ} $C during the cavity cooldown from 800 $^{\circ}$C and held at 165 $^{\circ}$C, without any degradation in accelerating gradient over the baseline performance. The treatment was applied to several elliptical cavities with frequency ranging from 0.75 GHz to 3.0 GHz, showing an improved quality factor as a result of low temperature nitrogen treatments. The Q-rise feature is similar to that achieved by nitrogen alloying Nb cavities at higher temperature, followed by material removal by electropolishing. The surface modification was confirmed by the change in electronic mean free path and tuned with the temperature and duration of heat treatment. The decrease of the temperature-dependent surface resistance with increasing RF field, resulting in a Q-rise, becomes stronger with increasing frequency and decreasing temperature. The data suggest a crossover frequency of $\sim 0.95$~GHz above which the Q-rise phenomenon occurs at 2~K. Some of these results can be explained qualitatively with an existing model of intrinsic field-dependence of the surface resistance with both equilibrium and nonequilibrium quasiparticle distribution functions. The change in the Q-slope below 0.95 GHz may result from masking contribution of trapped magnetic flux to the residual surface resistance.",2402.17458v3 2010-05-10,Advances in the Development of Micropattern Gaseous Detectors with Resistive Electrodes,"We describe the most recent efforts made by various groups in implementing resistive electrodes in micropattern gaseous detectors with the aim to combine in the same design the best features of RPCs (for the example, their robustness and spark protection property) with the high granularity and thus the good position resolution offered by microelectronic technology. In the stream of this activity, we have recently developed two novel detectors with resistive electrodes: one was based on resistive micromeshes and the second one is a MSGC with resistive electrodes. We have demonstrated that the resistive meshes are a convenient construction element for various designs of spark protective detectors: RPCs type, GEM type and MICROMEGAS type. These new detectors enable to considerably enhance the RPC and micropattern detectors applications since they feature not only a high position resolution but also a relatively good energy resolution (25-30 persent FWHM at 6 keV) and, if necessary, they can operate in cascaded mode allowing the achievement of a high overall gas gain. The main conclusion from these studies is that the implementation of resistive electrodes in micropattern detectors makes them fully spark protected; on this basis we consider this direction very promising.",1005.1477v1 2020-03-03,Filled Carbon Nanotubes as Anode Materials for Lithium-Ion Batteries,"Downsizing well-established materials to the nanoscale is a key route to novel functionalities, in particular if different functionalities are merged in hybrid nanomaterials. Hybrid carbon-based hierarchical nanostructures are particularly promising for electrochemical energy storage since they combine benefits of nanosize effects, enhanced electrical conductivity and integrity of bulk materials. We show that endohedral multiwalled carbon nanotubes (CNT) encapsulating high-capacity (here: conversion and alloying) electrode materials have a high potential for use in anode materials for lithium-ion batteries (LIB). There are two essential characteristics of filled CNT relevant for application in electrochemical energy storage: (1) rigid hollow cavities of the CNT provide upper limits for nanoparticles in their inner cavities which are both separated from the fillings of other CNT and protected against degradation. In particular, the CNT shells resist strong volume changes of encapsulates in response to electrochemical cycling, which in conventional conversion and alloying materials hinders application in energy storage devices. (2) Carbon mantles ensure electrical contact to the active material as they are unaffected by potential cracks of the encapsulate and form a stable conductive network in the electrode compound. Our studies confirm that encapsulates are electrochemically active and can achieve full theoretical reversible capacity. The results imply that encapsulating nanostructures inside CNT can provide a route to new high-performance nanocomposite anode materials for LIB.",2003.01379v1 2014-10-16,Electron beam induced current in the high injection regime,"Electron beam induced current (EBIC) is a powerful technique which measures the charge collection efficiency of photovoltaics with sub-micron spatial resolution. The exciting electron beam results in a high generation rate density of electron-hole pairs, which may drive the system into nonlinear regimes. An analytic model is presented which describes the EBIC response when the {\it total} electron-hole pair generation rate exceeds the rate at which carriers are extracted by the photovoltaic cell, and charge accumulation and screening occur. The model provides a simple estimate of the onset of the high injection regime in terms of the material resistivity and thickness, and provides a straightforward way to predict the EBIC lineshape in the high injection regime. The model is verified by comparing its predictions to numerical simulations in 1 and 2 dimensions. Features of the experimental data, such as the magnitude and position of maximum collection efficiency versus electron beam current, are consistent with the 3 dimensional model.",1410.4435v1 2018-04-09,Self-Modulation Doping Effect in the High-Mobility Layered Semiconductor Bi2O2Se,"Recently an air-stable layered semiconductor Bi2O2Se was discovered to exhibit an ultrahigh mobility in transistors fabricated with its thin layers. In this work, we explored the mechanism that induces the high mobility and distinguishes Bi2O2Se from other semiconductors. We found that the electron donor states lie above the lowest conduction band. Thus, electrons get spontaneously ionized from donor sites (e.g., Se vacancies) without involving the thermal activation, different from the donor ionization in conventional semiconductors. Consequently, the resistance decreases as reducing the temperature as observed in our measurement, which is similar to a metal but contrasts to a usual semiconductor. Furthermore, the electron conduction channels locate spatially away from ionized donor defects (Se vacancies) in different van der Waals layers. Such a spatial separation can strongly suppress the scattering caused by donor sites and subsequently increase the electron mobility, especially at the low temperature. We call this high-mobility mechanism self-modulation doping, i.e. the modulation doping spontaneously happening in a single-phase material without requiring a heterojunction. Our work paves a way to design novel high-mobility semiconductors with layered materials.",1804.03186v1 2019-05-21,Persistent antiferromagnetic order in heavily overdoped Ca$_{1-x}$La$_x$FeAs$_2$,"In the Ca$_{1-x}$La$_x$FeAs$_2$ (112) family of pnictide superconductors, we have investigated a highly overdoped composition (x = 0.56), prepared by high-pressure, high-temperature synthesis. Magnetic measurements show an antiferromagnetic transition at TN = 120K, well above the one at lower doping (0.15 < x < 0.27). Below the onset of long-range magnetic order at TN, the electrical resistivity is strongly reduced and is dominated by electron-electron interactions, as evident from its temperature dependence. The Seebeck coefficient shows a clear metallic behavior as in narrow band conductors. The temperature dependence of the Hall coefficient and the violation of Kohler's rule agree with the multiband character of the material. No superconductivity was observed down to 1.8 K. The success of the high-pressure synthesis encourages further investigations of the so far only partially explored phase diagram in this family of Iron-based high temperature superconductors.",1905.08640v1 2019-09-10,"Low temperature deformation of MoSi$_2$ and the effect of Ta, Nb and Al as alloying elements","Molybdenum disilicide (MoSi$_2$) is a very promising material for high temperature structural applications due to its high melting point (2030 {\deg}C), low density, high thermal conductivity and good oxidation resistance. However, MoSi$_2$ has limited ductility below 900 {\deg}C due to its anisotropic plastic deformation behaviour and high critical resolved shear stresses on particular slip systems. Nanoindentation of MoSi$_2$ microalloyed with aluminium, niobium or tantalum showed that all alloying elements cause a decrease in hardness. Analysis of surface slip lines indicated the activation of the additional {1 1 0}<1 1 1> slip system in microalloyed MoSi$_2$, which is not active below 300 {\deg}C in pure MoSi$_2$. This was confirmed by TEM dislocation analysis of the indentation plastic zone. Further micropillar compression experiments comparing pure MoSi$_2$ and the Ta-alloyed sample enabled the determination of the critical resolved shear stresses of individual slip systems even in the most brittle [0 0 1] crystal direction.",1909.04707v1 2017-07-06,A General Perspective of Fe-Mn-Al-C Steels,"During the last years, the scientific and industrial community has focused on the astonishing properties of Fe-Mn-Al-C steels. These high advanced steels allow high-density reductions about ~15% lighter than conventional steels, high corrosion resistance, high strength (ultimate tensile strength (UTS) ~1 Gpa) and at the same time ductilities above 60%. The increase of the tensile or yield strength and the ductility at the same time is almost a special feature of this kind of new steels, which makes them so interesting for many applications such as in the automotive, armor and mining industry. The control of these properties depends on a complex relationship between the chemical composition of the steel, the test temperature, the external loads and the processing parameters of the steel. This review has been conceived to tried to elucidate these complex relations and gather the most important aspects of Fe-Mn-Al-C steels developed so far.",1707.01920v2 2022-01-11,Fishtail effect and the vortex phase diagram of high-entropy alloy superconductor,"High-entropy alloy (HEA) is an attracting topic raising in materials science and condensed matter physics. Although several types of superconductors have been discovered in HEAs, the critical currents (Jc) of HEA superconductors remain uncharacterized up to now. Here, we systematically study the current-carrying ability of (TaNb)0.7(HfZrTi)0.5 HEA at various heat treatment conditions. We obtained the high upper critical field and large current carrying ability, which point to optimistic applications. Interestingly, the fishtail or second peak effect was found for the first time in HEA superconductors, and the position of the vortex pinning force shows a maximum at 0.72 of the reduced field, which is quite different from the cuprates and iron-based high-Tc superconductors. Together with the resistive measurements, the vortex phase diagram is obtained for HEA superconductor.",2201.03994v1 2023-01-12,Non-centrosymmetric Sr$_{2}$IrO$_{4}$ obtained under High Pressure,"Sr$_{2}$IrO$_{4}$ with strong spin-orbit coupling (SOC) and Hubbard repulsion (U) hosts Mott insulating states. The similar crystal structure, magnetic and electronic properties, particularly the $d$-wave gap observed in Sr$_{2}$IrO$_{4}$ enhanced the analogies to cuprate high-$T_{c}$ superconductor, La$_{2}$CuO$_{4}$. The incomplete analogy was due to the lack of broken inversion symmetry phases observed in Sr$_{2}$IrO$_{4}$. Here, under high pressure and high temperature conditions, we report a non-centrosymmetric Sr$_{2}$IrO$_{4}$. The crystal structure and its noncentrosymmetric character were determined by single crystal X-ray diffraction and high-resolution scanning transmission electron microscopy (HR-STEM). The magnetic characterization confirms the Ir$^{4+}$ with $S$ = 1/2 at low temperature in Sr$_{2}$IrO$_{4}$ with magnetic ordering occurred at around 86 K, where a larger moment is observed than the ambient pressure Sr$_{2}$IrO$_{4}$. Moreover, the resistivity measurement shows three-dimensional Mott variable-range hopping existed in the system. This non-centrosymmetric Sr$_{2}$IrO$_{4}$ phase appears to be a unique material to offer further understanding of high-$T_{c}$ superconductivity.",2301.05282v1 2010-12-31,Processing and study of the composite CdS/Bi-Pb-Sr-Ca-Cu-O,"We have fabricated and characterized samples of the superconducting- semiconducting Bi-Pb-Sb-Sr-Ca-Cu-O/CdS composite. Nano-size particles of CdS were deposited and introduced into the porosities of the Bi-Pb-Sb-Sr-Ca-Cu-O material by the spray pyrolysis technique. The morphology and hollow size in the porous superconducting material as well as the grain size in CdS and the morphology of the surface of the composite were obtained by Scanning Electron Microscopy. We obtained the critical superconducting temperature of both the Bi-Pb-Sb-Sr-Ca-Cu-O and the Bi-Pb-Sb-Sr-Ca-Cu-O/CdS composite measuring the resistivity. Both show a metallic behaviour just above the superconducting transition. For the superconductor alone, resistivity starts falling at Tc,on sup = 99,9 K and reaches zero at Tc,sup=76,3 K. The behaviour of the composite is different. The transition starts at Tc,on comp = 65,3 K and reaches zero resistance at Tc,comp = 56,5 K. This seems to indicate that the semiconductor penetrates the whole superconducting Bi-Pb-Sb-Sr-Ca-Cu-O sample so that there is no region of pure superconducting material left. Since the materials do not actually mix (see text) the behaviour might be attributable to the interface. Also the resistivity curves present a very interesting feature, i.e., below the temperature at which the composite attains zero-resistivity, a re-entrant behaviour manifests itself and a finite resistivity peak appears. It increases to a certain value to drop back to zero at some temperature below. We comment further on this feature in the text.",1101.0277v1 2009-02-02,"Single crystals of LnFeAsO1-xFx (Ln=La, Pr, Nd, Sm, Gd) and Ba1-xRbxFe2As2: growth, structure and superconducting properties","A review of our investigations on single crystals of LnFeAsO1-xFx (Ln=La, Pr, Nd, Sm, Gd) and Ba1-xRbxFe2As2 is presented. A high pressure technique has been applied for the growth of LnFeAsO1-xFx crystals, while Ba1-xRbxFe2As2 crystals were grown using quartz ampoule method. Single crystals were used for electrical transport, structure, magnetic torque and spectroscopic studies. Investigations of the crystal structure confirmed high structural perfection and show less than full occupation of the (O, F) position in superconducting LnFeAsO1-xFx crystals. Resistivity measurements on LnFeAsO1-xFx crystals show a significant broadening of the transition in high magnetic fields, whereas the resistive transition in Ba1 xRbxFe2As2 simply shifts to lower temperature. Critical current density for both compounds is relatively high and exceeds 2x109 A/m2 at 15 K in 7 T. The anisotropy of magnetic penetration depth, measured on LnFeAsO1-xFx crystals by torque magnetometry is temperature dependent and apparently larger than the anisotropy of the upper critical field. Ba1-xRbxFe2As2 crystals are electronically significantly less anisotropic. Point-Contact Andreev-Reflection spectroscopy indicates the existence of two energy gaps in LnFeAsO1-xFx. Scanning Tunneling Spectroscopy reveals in addition to a superconducting gap, also some feature at high energy (~20 meV).",0902.0224v2 2020-03-20,"Anisotropy of the transport properties of NdFeAs(O,F) thin films grown on vicinal substrates","NdFeAs(O,F) thin films having different fluorine contents were grown on 5 deg. or 10 deg. vicinal cut MgO and CaF2 single crystalline substrates by molecular beam epitaxy. Structural characterisations by reflection high-energy electron diffraction and x-ray diffraction confirmed the epitaxial growth of NdFeAs(O,F). The resistivities of the ab-plane and along the c-axis were derived from the resistivity measurements in the longitudinal and transversal directions. The c-axis resistivity was always higher than the ab-plane resistivity, resulting from the anisotropic electronic structure. The resistivity anisotropy at 300 K was almost constant in the range of 50-90 irrespective of the F content. On the other hand, the resistivity anisotropy at 56 K showed a strong fluorine dependence: the resistivity anisotropy was over 200 for the films with optimum F contents (superconducting transition temperature Tc around 50 K), whereas the resistivity anisotropy was around 70 for the films in the under-doped regime (Tc between 35 and 45 K). The mass anisotropy are the effective masses along the c-axis and on the ab-plane) close to Tc derived from the anisotropic Ginzburg-Landau approach using the angular-dependency of the ab-plane resistivity was in the range from 2 to 5. On the assumption that the square of the mass anisotropy is equal to the resistivity anisotropy, those values are small compared to the normal state anisotropy.",2003.09105v1 2017-03-23,Development and characterization of Brassica juncea fruticulosa introgression lines exhibiting resistance to mustard aphid,"Background: Mustard aphid is a major pest of Brassica oilseeds. No source for aphid resistance is presently available in Brassica juncea . A wild crucifer, Brassica fruticulosa is known to be resistant to mustard aphid. An artificially synthesized amphiploid, AD-4 (B. fruticulosa x B. rapa var. brown sarson) was developed for use as a bridge species to transfer fruticulosa resistance to B. juncea. Using the selfed backcross we could select a large number of lines with resistance to mustard aphid. This paper reports cytogenetic stability of introgression lines, molecular evidence for alien introgression and their reaction to mustard aphid infestation. Results: Majority of introgression lines had expected euploid chromosome number(2n= 36), showed normal meiosis and high pollen grain fertility. Well-distributed and transferable simple-sequence repeats (SSR) markers for all the 18 B. juncea chromosomes helped to characterize introgression events. Average proportions of recipient and donor genome in the substitution lines were 49.72 and 35.06%, respectively. Minimum alien parent genome presence (27.29%) was observed in the introgression line, Ad3K-280 . Introgressed genotypes also varied for their resistance responses to mustard aphid infestations under artificial release conditions for two continuous seasons. Some of the test genotypes showed consistent resistant reaction. Conclusions: B.juncea-fruticulosa introgression set may prove to be a very powerful breeding tool for aphid resistance related QTL/gene discovery and fine mapping of the desired genes/QTLs to facilitate marker assisted transfer of identified gene(s) for mustard aphid resistance in the background of commercial mustard genotypes.",1703.07987v1 2020-09-21,Chaos-induced resistivity in different magnetic configurations,"It is widely believed that magnetic reconnection plays an important role in various eruptive phenomena of space and astrophysical plasmas. The mechanism of anomalous resistivity, however, has been an open and unsolved problem. The chaos-induced resistivity proposed by Yoshida (1998) is one of possible mechanisms for anomalous resistivity. By use of the test particle simulation, the present work studies the chaos-induced resistivity for different configurations of reconnection magnetic fields and its distribution in different chaos regions of reconnection current sheets. The results show that the chaos-induced resistivity can be 6-7 orders of magnitude higher than the classical Spitzer resistivity in the X-type chaos regions and 5 orders of magnitude in the O-type chaos regions. Moreover, in the X-type chaos regions the chaos-induced resistivity of the magnetized case is higher by a factor of 2 to 3 times than that of the unmagnetized case, but in the O-type chaos regions the chaos-induced resistivity of the magnetized case is close to or lower than that of the unmagnetized case. The present work is helpful to the understanding of the dynamics of reconnection current sheets, especially of the generation mechanism of the anomalous resistivity of collisionless reconnection regions.",2009.09745v1 2019-12-10,Temperature and gate effects on contact resistance and mobility in graphene transistors by TLM and Y-function methods,"The metal-graphene contact resistance is one of the major limiting factors toward the technological exploitation of graphene in electronic devices and sensors. A high contact resistance can be detrimental to device performance and spoil the intrinsic great properties of graphene. In this paper, we fabricate graphene field-effect transistors with different geometries to study the contact and channel resistance as well as the carrier mobility as a function of gate voltage and temperature. We apply the transfer length method and the y-function method showing that the two approaches can complement each other to evaluate the contact resistance and prevent artifacts in the estimation of the gate-voltage dependence of the carrier mobility. We find that the gate voltage modulates the contact and the channel resistance in a similar way but does not change the carrier mobility. We also show that the raising temperature lowers the carrier mobility, has negligible effect on the contact resistance, and can induce a transition from a semiconducting to a metallic behavior of the graphene sheet resistance, depending on the applied gate voltage. Finally we show that eliminating the detrimental effects of the contact resistance on the transistor channel current almost doubles the carrier field-effect mobility and that a competitive contact resistance an be achieved by the zig-zag shaping of the Ni contact.",1912.04623v1 2019-12-17,Mitigate Parasitic Resistance in Resistive Crossbar-based Convolutional Neural Networks,"Traditional computing hardware often encounters on-chip memory bottleneck on large scale Convolution Neural Networks (CNN) applications. With its unique in-memory computing feature, resistive crossbar-based computing attracts researchers' attention as a promising solution to the memory bottleneck issue in von Neumann architectures. However, the parasitic resistances in the crossbar deviate its behavior from the ideal weighted summation operation. In large-scale implementations, the impact of parasitic resistances must be carefully considered and mitigated to ensure circuits' functionality. In this work, we implemented and simulated CNNs on resistive crossbar circuits with consideration of parasitic resistances. Moreover, we carried out a new mapping scheme for high utilization of crossbar arrays on convolution, and a mitigation algorithm to mitigate parasitic resistances in CNN applications. The mitigation algorithm considers parasitic resistances as well as data/kernel patterns of each layer to minimize the computing error in crossbar-based convolutions of CNNs. We demonstrated the proposed methods with implementations of a 4-layer CNN on MNIST and ResNet(20, 32, and 56) on CIFAR-10. Simulation results show the proposed methods well mitigate the parasitic resistances in crossbars. With our methods, modern CNNs on crossbars can preserve ideal(software) level classification accuracy with 6-bit ADCs and DACs implementation.",1912.08716v1 2017-03-23,Influence of material parameters on the performance of niobium based superconducting RF cavities,"A detailed thermal analysis of a Niobium (Nb) based superconducting radio frequency (SRF) cavity in a liquid helium bath is presented, taking into account the temperature and magnetic field dependence of the surface resistance and thermal conductivity in the superconducting state of the starting Nb material (for SRF cavity fabrication) with different impurity levels. The drop in SRF cavity quality factor (Q_0) in the high acceleration gradient regime (before ultimate breakdown of the SRF cavity) is studied in details. It is argued that the high field Q_0-drop in SRF cavity is considerably influenced by the intrinsic material parameters such as electrical conductivity, and thermal diffusivity. The detail analysis also shows that the current specification on the purity of niobium material for SRF cavity fabrication is somewhat over specified. Niobium material with a relatively low purity can very well serve the purpose for the accelerators dedicated for spallation neutron source (SNS) or accelerator driven sub-critical system (ADSS) applications, where the required accelerating gradient is typically up to 20 MV/m,. This information will have important implication towards the cost reduction of superconducting technology based particle accelerators for various applications.",1703.07985v3 2015-01-09,Superconductivity in quasi-one-dimensional Cs2Cr3As3 with large interchain distance,"Since the discovery of high-temperature superconductivity (SC) in quasi-two-dimensional copper oxides, a few layered compounds, which bear similarities to the cuprates, have also been found to host unconventional SC. Our recent observation of SC at 6.1 K in correlated electron material K2Cr3As3 (J. K. Bao et al., arXiv: 1412.0067) represents an obviously different paradigm, primarily because of its quasi-one-dimensional (Q1D) nature. The new material is structurally featured by the (Cr3As3)2- double-walled subnano-tubes composed of face-sharing Cr6/2 (As6/2) octahedron linear chains, which are well separated by columns of K+ counterions. Later, an isostructural superconducting Rb2Cr3As3 was synthesized, thus forming a new superconducting family. Here we report the third member, Cs2Cr3As3, which possesses the largest interchain distance. SC appears below 2.2 K. Similar to the former two sister compounds, Cs2Cr3As3 exhibits a non-Fermi liquid behavior with a linear temperature dependence of resistivity in the normal state, and a high upper critical field beyond the Pauli limit as well, suggesting common unconventional SC in the Q1D Cr-based material.",1501.02065v1 2018-03-05,Simulation study of ballistic spin-MOSFET devices with ferromagnetic channels based on some Heusler and oxide compounds,"Newly emerged materials from the family of Heuslers and complex oxides exhibit finite bandgaps and ferromagnetic behavior with Curie temperatures much higher than even room temperature. In this work, using the semiclassical top-of-the-barrier FET model, we explore the operation of a spin-MOSFET that utilizes such ferromagnetic semiconductors as channel materials, in addition to ferromagnetic source/drain contacts. Such a device could retain the spin polarization of injected electrons in the channel, the loss of which limits the operation of traditional spin transistors with non-ferromagnetic channels. We examine the operation of four material systems that are currently considered some of the most prominent known ferromagnetic semiconductors, three Heusler-type alloys (Mn2CoAl, CrVZrAl, CoVZrAl) and one from the oxide family (NiFe2O4). We describe their bandstructures by using data from DFT calculations. We investigate under which conditions high spin polarization and significant ION/IOFF ratio, two essential requirements for the spin-MOSFET operation, are both achieved. We show that these particular Heusler channels, in their bulk form, do not have adequate bandgap to provide high ION/IOFF ratios, and have small magnetoconductance compared to state-of-the-art devices. However, with confinement into ultra-narrow sizes down to a few nanometers, and by engineering their spin dependent contact resistances, they could prove promising channel materials for the realization of spin-MOSFET transistor devices that offer combined logic and memory functionalities. Although the main compounds of interest in this paper are Mn2CoAl, CrVZrAl, CoVZrAl, and NiFe2O4 alone, we expect that the insight we provide is relevant to other classes of such materials as well.",1803.01789v1 2022-03-14,HDPView: Differentially Private Materialized View for Exploring High Dimensional Relational Data,"How can we explore the unknown properties of high-dimensional sensitive relational data while preserving privacy? We study how to construct an explorable privacy-preserving materialized view under differential privacy. No existing state-of-the-art methods simultaneously satisfy the following essential properties in data exploration: workload independence, analytical reliability (i.e., providing error bound for each search query), applicability to high-dimensional data, and space efficiency. To solve the above issues, we propose HDPView, which creates a differentially private materialized view by well-designed recursive bisected partitioning on an original data cube, i.e., count tensor. Our method searches for block partitioning to minimize the error for the counting query, in addition to randomizing the convergence, by choosing the effective cutting points in a differentially private way, resulting in a less noisy and compact view. Furthermore, we ensure formal privacy guarantee and analytical reliability by providing the error bound for arbitrary counting queries on the materialized views. HDPView has the following desirable properties: (a) Workload independence, (b) Analytical reliability, (c) Noise resistance on high-dimensional data, (d) Space efficiency. To demonstrate the above properties and the suitability for data exploration, we conduct extensive experiments with eight types of range counting queries on eight real datasets. HDPView outperforms the state-of-the-art methods in these evaluations.",2203.06791v3 2024-01-23,Integration of High-Tc Superconductors with High Q Factor Oxide Mechanical Resonators,"Micro-mechanical resonators are building blocks of a variety of applications in basic science and applied electronics. This device technology is mainly based on well-established and reproducible silicon-based fabrication processes with outstanding performances in term of mechanical Q factor and sensitivity to external perturbations. Broadening the functionalities of MEMS by the integration of functional materials is a key step for both applied and fundamental science. However, combining functional materials and silicon-based compounds is challenging. An alternative approach is fabricating MEMS based on complex heterostructures made of materials inherently showing a variety of physical properties such as transition metal oxides. Here, we report on the integration of a high-Tc superconductor YBa2Cu3O7 (YBCO) with high Q factor micro-bridge resonator made of a single-crystal LaAlO3 (LAO) thin film. LAO resonators are tensile strained, with a stress of 345 MPa, show Q factor in the range of tens of thousands, and have low roughness. The topmost YBCO layer deposited by Pulse Laser Deposition shows a superconducting transition starting at 90 K with zero resistance below 78 K. This result opens new possibilities towards the development of advanced transducers, such as bolometers or magnetic field detectors, as well as basic science experiments in solid state physics, material science, and quantum opto-mechanics.",2401.12758v1 2004-06-25,Resistance Noise Near to Electrical Breakdown: Steady State of Random Networks as a Function of the Bias,"A short review is presented of a recently developed computational approach which allows the study of the resistance noise over the full range of bias values, from the linear regime up to electrical breakdown. Resistance noise is described in terms of two competing processes in a random resistor network. The two processes are thermally activated and driven by an electrical bias. In the linear regime, a scaling relation has been found between the relative variance of resistance fluctuations and the average resistance. The value of the critical exponent is significantly higher than that associated with 1/f noise. In the nonlinear regime, occurring when the bias overcomes the threshold value, the relative variance of resistance fluctuations scales with the bias. Two regions can be identified in this regime: a moderate bias region and a pre-breakdown one. In the first region, the scaling exponent has been found independent of the values of the model parameters and of the bias conditions. A strong nonlinearity emerges in the pre-breakdown region which is also characterized by non-Gaussian noise. The results compare well with measurements of electrical breakdown in composites and with electromigration experiments in metallic lines.",0406648v1 2010-11-29,"Contact effects on transport in magnetite, an archetypal correlated transition metal oxide","Multiterminal measurements have typically been employed to examine electronic properties of strongly correlated electronic materials such as transition metal oxides without the influence of contact effects. In contrast, in this work we investigate the interface properties of Fe$_3$O$_4$ with different metals, with the contact effects providing a window on the physics at work in the correlated oxide. Contact resistances are determined by means of four-terminal electrical measurements as a function of source voltage and temperature. Contact resistances vary systematically with the work function of the electrode metal, $\phi(M)$, $M=$Cu, Au and Pt, with higher work function yielding lower contact resistance. This trend and the observation that contact resistances are directly proportional to the Fe$_3$O$_4$ resistivity are consistent with modeling the oxide as an effective $p$-type semiconductor with hopping transport. The jumps in contact resistance values at the bias-driven insulator-metal transition have a similar trend with $\phi$($M$), consistent with the transition mechanism of charge gap closure by electric field.",1011.6407v1 2012-10-01,Thermal Contact Resistance Across Nanoscale Silicon Dioxide and Silicon Interface,"Silicon dioxide and silicon (SiO$_{2}$/Si) interface plays a very important role in semiconductor industry. However, at nanoscale, its interfacial thermal properties haven't been well understood so far. In this paper, we systematically study the interfacial thermal resistance (Kapitza resistance) of a heterojunction composed of amorphous silicon dioxide and crystalline silicon by using molecular dynamics simulations. Numerical results have shown that Kapitza resistance at SiO$_{2}$/Si interface depends on the interfacial coupling strength remarkably. In the weak interfacial coupling limit, Kapitza resistance depends on both the detailed interfacial structure and the length of the heterojunction, showing large fluctuation among different samples. In contrast, it is almost insensitive to the detailed interfacial structure or the length of the heterojunction in the strong interfacial coupling limit, giving rise to a nearly constant value around 0.9 $\times10^{-9}$ m$^{2}$KW$^{-1}$ at room temperature. Moreover, the temperature dependent Kapitza resistance in the strong interfacial coupling limit has also been examined. Our study provides useful guidance to the thermal management and heat dissipation across nanoscale SiO$_{2}$/Si interface, in particular for the design of silicon nanowire based nano electronics and photonics devices.",1210.0354v1 2013-02-19,Local breakdown of the quantum Hall effect in narrow single layer graphene Hall devices,"We have analyzed the breakdown of the quantum Hall effect in 1 micrometer wide Hall devices fabricated from an exfoliated monolayer graphene transferred on SiOx. We have observed that the deviation of the Hall resistance from its quantized value is weakly dependent on the longitudinal resistivity up to current density of 5 A/m, where the Hall resistance remains quantized even when the longitudinal resistance increases monotonously with the current. Then a collapse in the quantized resistance occurs while longitudinal resistance keeps its gradual increase. The exponential increase of the conductivity with respect to the current suggests impurity mediated inter-Landau level scattering as the mechanism of the breakdown. The results are interpreted as the strong variation of the breakdown behavior throughout the sample due to the randomly distributed scattering centers that mediates the breakdown.",1302.4729v1 2016-01-17,Low-resistance GaN tunnel homojunctions with 150 kA/cm^2 current and repeatable negative differential resistance,"We report GaN n++/p++ interband tunnel junctions with repeatable negative differential resistance and low resistance. Reverse and forward tunneling current densities were observed to increase as Si and Mg doping concentrations were increased. Hysteresis-free, bidirectional negative differential resistance was observed at room temperature from these junctions at a forward voltage of ~1.6-2 V. Thermionic PN junctions with tunnel contact to the p-layer exhibited forward current density of 150 kA/cm^2 at 7.6 V, with a low series device resistance of 1 x 10^-5 ohm.cm^2.",1601.04353v2 2017-02-13,Deconstructing temperature gradients across fluid interfaces: the structural origin of the thermal resistance of liquid-vapor interfaces,"The interfacial thermal resistance determines condensation-evaporation processes and thermal transport across material-fluid interfaces. Despite its importance in transport processes, the interfacial structure responsible for the thermal resistance is still unknown. By combining non-equilibrium molecular dynamics simulations and interfacial analyses that remove the interfacial thermal fluctuations we show that the thermal resistance of liquid-vapor interfaces is connected to a low density fluid layer that is adsorbed at the liquid surface. This thermal resistance layer (TRL) defines the boundary where the thermal transport mechanism changes from that of gases (ballistic) to that characteristic of dense liquids, dominated by frequent particle collisions involving very short mean free paths. We show that the thermal conductance is proportional to the number of atoms adsorbed in the TRL, and hence we explain the structural origin of the thermal resistance in liquid-vapor interfaces.",1702.03896v2 2018-03-21,Measuring the thermal conductivity and interfacial thermal resistance of suspended MoS2 using electron beam self-heating technique,"Establishment of a new technique or extension of an existing technique for thermal and thermoelectric measurements to a more challenging system is an important task to explore the thermal and thermoelectric properties of various materials and systems. The bottleneck lies in the challenges in measuring the thermal contact resistance. In this work, we applied electron beam self-heating technique to derive the intrinsic thermal conductivity of suspended Molybdenum Disulfide (MoS2) ribbons and the thermal contact resistance, with which the interfacial thermal resistance between few-layer MoS2 and Pt electrodes was calculated. The measured room temperature thermal conductivity of MoS2 is around 30 W/mK, while the estimated interfacial thermal resistance is around 2*10-6 m2K/W. Our experiments extend a useful branch in application of this technique for studying thermal properties of suspended layered ribbons and have potential application in investigating the interfacial thermal resistance of different 2D heterojunctions.",1803.07757v1 2019-09-16,An experimental proof that resistance-switching memories are not memristors,"It has been suggested that all resistive-switching memory cells are memristors. The latter are hypothetical, ideal devices whose resistance, as originally formulated, depends only on the net charge that traverses them. Recently, an unambiguous test has been proposed [J. Phys. D: Appl. Phys. {\bf 52}, 01LT01 (2019)] to determine whether a given physical system is indeed a memristor or not. Here, we experimentally apply such a test to both in-house fabricated Cu-SiO2 and commercially available electrochemical metallization cells. Our results unambiguously show that electrochemical metallization memory cells are not memristors. Since the particular resistance-switching memories employed in our study share similar features with many other memory cells, our findings refute the claim that all resistance-switching memories are memristors. They also cast doubts on the existence of ideal memristors as actual physical devices that can be fabricated experimentally. Our results then lead us to formulate two memristor impossibility conjectures regarding the impossibility of building a model of physical resistance-switching memories based on the memristor model.",1909.07238v2 2014-08-22,"Resistance and lifetime measurements of polymer solar cells using glycerol doped poly[3,4-ethylenedioxythiophene]: poly[styrenesulfonate] hole injection layers","We have performed resistivity measurements of poly[3,4-ethylenedioxythiophene]: poly[styrenesulfonate] (PEDOT:PSS) films with varying concentrations of glycerol. Resistivity is seen to decrease exponentially from roughly 3 ohm-cm for pure PEDOT:PSS to 3x10-2 ohm-cm for 35 mg/cm3 glycerol in PEDOT:PSS. Beyond this concentration adding glycerol does not significantly change resistivity. Bulk heterojunction polymer solar cells using these variously doped PEDOT:PSS layers as electrodes were studied to characterize the effects on efficiency and lifetime. Although our data display significant scatter, lowering the resistance of the PEDOT:PSS layers results in lower device resistance and higher efficiency as expected. We also note that the lifetime of the devices tends to be reduced as the glycerol content of PEDOT:PSS is increased. Many devices show an initial increase in efficiency followed by a roughly exponential decay. This effect is explained based on concomitant changes in the zero bias conductance of the samples under dark conditions.",1408.5199v2 2017-01-17,Grain Boundary Resistance in Copper Interconnects from an Atomistic Model to a Neural Network,"Orientation effects on the resistivity of copper grain boundaries are studied systematically with two different atomistic tight binding methods. A methodology is developed to model the resistivity of grain boundaries using the Embedded Atom Model, tight binding methods and non-equilibrum Green's functions (NEGF). The methodology is validated against first principles calculations for small, ultra-thin body grain boundaries (<5nm) with 6.4% deviation in the resistivity. A statistical ensemble of 600 large, random structures with grains is studied. For structures with three grains, it is found that the distribution of resistivities is close to normal. Finally, a compact model for grain boundary resistivity is constructed based on a neural network.",1701.04897v3 2015-07-20,Effect of Covalent Functionalisation on Thermal Transport Across Graphene-Polymer Interfaces,"This paper is concerned with the interfacial thermal resistance for polymer composites reinforced by various covalently functionalised graphene. By using molecular dynamics simulations, the obtained results show that the covalent functionalisation in graphene plays a significant role in reducing the graphene-paraffin interfacial thermal resistance. This reduction is dependent on the coverage and type of functional groups. Among the various functional groups, butyl is found to be the most effective in reducing the interfacial thermal resistance, followed by methyl, phenyl and formyl. The other functional groups under consideration such as carboxyl, hydroxyl and amines are found to produce negligible reduction in the interfacial thermal resistance. For multilayer graphene with a layer number up to four, the interfacial thermal resistance is insensitive to the layer number. The effects of the different functional groups and the layer number on the interfacial thermal resistance are also elaborated using the vibrational density of states of the graphene and the paraffin matrix. The present findings provide useful guidelines in the application of functionalised graphene for practical thermal management.",1507.05397v1 2020-12-05,Machine Learning and Data Analytics for Design and Manufacturing of High-Entropy Materials Exhibiting Mechanical or Fatigue Properties of Interest,"This chapter presents an innovative framework for the application of machine learning and data analytics for the identification of alloys or composites exhibiting certain desired properties of interest. The main focus is on alloys and composites with large composition spaces for structural materials. Such alloys or composites are referred to as high-entropy materials (HEMs) and are here presented primarily in context of structural applications. For each output property of interest, the corresponding driving (input) factors are identified. These input factors may include the material composition, heat treatment, manufacturing process, microstructure, temperature, strain rate, environment, or testing mode. The framework assumes the selection of an optimization technique suitable for the application at hand and the data available. Physics-based models are presented, such as for predicting the ultimate tensile strength (UTS) or fatigue resistance. We devise models capable of accounting for physics-based dependencies. We factor such dependencies into the models as a priori information. In case that an artificial neural network (ANN) is deemed suitable for the applications at hand, it is suggested to employ custom kernel functions consistent with the underlying physics, for the purpose of attaining tighter coupling, better prediction, and for extracting the most out of the - usually limited - input data available.",2012.07583v1 2000-11-10,The origin of high transport spin polarization in La$_{0.7}$Sr$_{0.3} $MnO$_{3}$: direct evidence for minority spin states,"Using the point contact Andreev reflection technique, we have carried out a systematic study of the spin polarization in the colossal magnetoresistive manganite, La$_{0.7}$Sr$_{0.3}$MnO$_{3}$} (LSMO). Surprisingly, we observed a significant increase in the current spin polarization with the residual resistivity. This counterintuitive trend can be understood as a transition from ballistic to diffusive transport in the contact. Our results strongly suggest that LSMO does have minority spin states at the Fermi level. However, since its current spin polarization is much higher than that of the density of states, this material can mimic the behavior of a true half-metal in transport experiments. Based on our results we call this material a {\it transport} half-metal.",0011198v1 2006-05-30,Complex Precipitation Pathways in Multi-Component Alloys,"One usual way to strengthen a metal is to add alloying elements and to control the size and the density of the precipitates obtained. However, precipitation in multicomponent alloys can take complex pathways depending on the relative diffusivity of solute atoms and on the relative driving forces involved. In Al-Zr-Sc alloys, atomic simulations based on first-principle calculations combined with various complementary experimental approaches working at different scales reveal a strongly inhomogeneous structure of the precipitates: owing to the much faster diffusivity of Sc compared with Zr in the solid solution, and to the absence of Zr and Sc diffusion inside the precipitates, the precipitate core is mostly Sc-rich, whereas the external shell is Zr-rich. This explains previous observations of an enhanced nucleation rate in Al-Zr-Sc alloys compared with binary Al-Sc alloys, along with much higher resistance to Ostwald ripening, two features of the utmost importance in the field of light high-strength materials.",0605738v1 2006-11-06,Coexisting tuneable fractions of glassy and equilibrium long-range-order phases in manganites,"Antiferromagnetic-insulating(AF-I) and the ferromagnetic-metallic(FM-M) phases coexist in various half-doped manganites over a range of temperature and magnetic field, and this is often believed to be an essential ingredient to their colossal magnetoresistence. We present magnetization and resistivity measurements on Pr(0.5)Ca(0.5)Mn(0.975)Al(0.025)O(3) and Pr(0.5)Sr(0.5)MnO(3) showing that the fraction of the two coexisting phases at low-temperature in any specified measuring field H, can be continuously controlled by following designed protocols traversing field-temperature space; for both materials the FM-M fraction rises under similar cooling paths. Constant-field temperature variations however show that the former sample undergoes a 1st order transition from AF-I to FM-M with decreasing T, while the latter undergoes the reverse transition. We suggest that the observed path-dependent phase-separated states result from the low-T equilibrium phase coexisting with supercooled glass-like high temperature phase, where the low-T equilibrium phases are actually homogeneous FM-M and AF-I phases respectively for the two materials.",0611152v1 2008-05-27,Colossal electroresistance effect around room temperature in LuFe2O4,"A colossal electroresistance effect is observed around room temperature in a transition metal oxide LuFe2O4. The measurements of resistance under various applied voltages as well as the highly nonlinear current-voltage characteristics reveal that a small electric field is able to drive the material from the insulating state to a metallic state. The threshold field at which the insulating-metallic transition occurs, decreases exponentially with increasing temperature. We interpret this transition as a consequence of the breakdown of the charge-ordered state triggered by applied electric field, which is supported by the dramatic dielectric response in a small electric field. This colossal electroresistance effect as well as the high dielectric tunability around room temperature in low applied fields makes LuFe2O4 a very promising material for many applications.",0805.4042v1 2008-07-21,Superconducting and thermal properties of ex-situ Glidcop sheathed multifilamentary MgB2 wires,"In DC and AC practical applications of MgB2 superconducting wires an important role is represented by the material sheath which has to provide, among other things, a suitable electrical and thermal stabilization. A way to obtain a large enough amount of low resistivity material in to the conductor architecture is to use it as external sheath. In this paper we study ex-situ multifilamentary MgB2 wires using oxide-dispersion-strengthened copper (GlidCop) as external sheath in order to reach a good compromise between critical current density and thermal properties. We prepared three GlidCop samples differing by the content of dispersed sub-microscopic Al2O3 particles. We characterized the superconducting and thermal properties and we showed that the good thermal conductivity together the good mechanical properties and a reasonable critical current density make of GlidCop composite wire a useful conductor for applications where high thermal conductivity is request at temperature above 30K, such as Superconducting-FCL.",0807.3259v1 2012-12-14,Using metallic photonic crystals as visible light sources,"In this paper we study numerically and experimentally the possibility of using metallic photonic crystals (PCs) of different geometries (log-piles, direct and inverse opals) as visible light sources. It is found that by tuning geometrical parameters of a direct opal PC one can achieve substantial reduction of the emissivity in the infrared along with its increase in the visible. We take into account disorder of the PC elements in their sizes and positions, and get quantitative agreement between the numerical and experimental results. We analyze the influence of known temperature-resistant refractory host materials necessary for fixing the PC elements, and find that PC effects become completely destroyed at high temperatures due to the host absorption. Therefore, creating PC-based visible light sources requires that low-absorbing refractory materials for embedding medium be found.",1212.3451v1 2013-01-10,Weak antilocalization in topological insulator Bi$_{2}$Te$_{3}$ microflakes,"We have studied the carrier transport in two topological insulator (TI) Bi$_{2}$Te$_{3}$ microflakes between 0.3 and 10 K and under applied backgate voltages ($V_{\rm BG}$). Logarithmic temperature dependent resistance corrections due to the two-dimensional electron-electron interaction effect in the presence of weak disorder were observed. The extracted Coulomb screening parameter is negative, which is in accord with the situation of strong spin-orbit scattering as is inherited in the TI materials. In particular, positive magnetoresistances (MRs) in the two-dimensional weak-antilocalization (WAL) effect were measured in low magnetic fields, which can be satisfactorily described by a multichannel-conduction model. Both at low temperatures of $T < 1$ K and under high positive $V_{\rm BG}$, signatures of the presence of two coherent conduction channels were observed, as indicated by an increase by a factor of $\approx$ 2 in the prefactor which characterizes the WAL MR magnitude. Our results are discussed in terms of the (likely) existence of the Dirac fermion surface states, in addition to the bulk states, in the three-dimensional TI Bi$_2$Te$_3$ material.",1301.2023v1 2013-12-12,Niobium Silicon alloys for Kinetic Inductance Detectors,"We are studying the properties of Niobium Silicon amorphous alloys as a candidate material for the fabrication of highly sensitive Kinetic Inductance Detectors (KID), optimized for very low optical loads. As in the case of other composite materials, the NbSi properties can be changed by varying the relative amounts of its components. Using a NbSi film with T_c around 1 K we have been able to obtain the first NbSi resonators, observe an optical response and acquire a spectrum in the band 50 to 300 GHz. The data taken show that this material has very high kinetic inductance and normal state surface resistivity. These properties are ideal for the development of KID. More measurements are planned to further characterize the NbSi alloy and fully investigate its potential.",1312.3588v1 2014-07-05,Approaching the Limits of Transparency and Conductivity in Graphitic Materials through Lithium Intercalation,"Various bandstructure engineering methods have been studied to improve the performance of graphitic transparent conductors; however none demonstrated an increase of optical transmittance in the visible range. Here we measure in situ optical transmittance spectra and electrical transport properties of ultrathin-graphite (3-60 graphene layers) simultaneously via electrochemical lithiation/delithiation. Upon intercalation we observe an increase of both optical transmittance (up to twofold) and electrical conductivity (up to two orders of magnitude), strikingly different from other materials. Transmission as high as 91.7% with a sheet resistance of 3.0 {\Omega} per square is achieved for 19-layer LiC6, which corresponds to a figure of merit {\sigma}_dc/{\sigma}_opt = 1400, significantly higher than any other continuous transparent electrodes. The unconventional modification of ultrathin-graphite optoelectronic properties is explained by the suppression of interband optical transitions and a small intraband Drude conductivity near the interband edge. Our techniques enable the investigation of other aspects of intercalation in nanostructures.",1407.1416v1 2014-10-02,Absence of the Ordinary and Extraordinary Hall effects scaling in granular ferromagnets at metal-insulator transition,"Universality of the extraordinary Hall effect scaling was tested in granular three-dimensional Ni-SiO2 films across the metal-insulator transition. Three types of magnetotransport behavior have been identified: metallic, weakly insulating and strongly insulating. Scaling between both the ordinary and extraordinary Hall effects and material resistivity is absent in the weakly insulating range characterized by logarithmic temperature dependence of conductivity. The results provide compelling experimental confirmation to recent models of granular metals predicting transition from logarithmic to exponential conductivity temperature dependence when inter-granular conductance drops below the quantum conductance value and loss of Hall effect scaling when inter-granular conductance is higher than the quantum one. The effect was found at high temperatures and reflects the granular structure of material rather than low temperature quantum corrections.",1410.0491v1 2014-11-04,Self-consistent modelling of nonlinear dynamic ESM microscopy in mixed ionic-electronic conductors,"Dynamic Electrochemical Strain Microscopy (ESM) response of mixed ionic-electronic conductors is analysed in the framework of the Thomas-Fermi screening theory and Vegard law with accounting of the steric effects. The emergence of dynamic charge waves and nonlinear deformation of the surface as result of applying probing voltage is numerically explored. 2D maps of the strain and concentration distribution across the mixed ionic-electronic conductor and bias-induced surface displacements for ESM microscopy were calculated. Obtained numerical results can be of applied to quantify ESM response of Li-based solid electroytes, materials with resistive switching and electroactive ferroelectric polymers, which are of potential interest for flexible and high-density non-volatile memory devices.",1411.0966v1 2015-06-03,Stable room-temperature ferromagnetic phase at the FeRh(100) surface,"Interfaces and low dimensionality are sources of strong modifications of electronic, structural, and magnetic properties of materials. FeRh alloys are an excellent example because of the first-order phase transition taking place at $\sim$400 K from an antiferromagnetic phase at room temperature to a high temperature ferromagnetic one. It is accompanied by a resistance change and volume expansion of about 1\%. We have investigated the electronic and magnetic properties of FeRh(100) epitaxially grown on MgO by combining spectroscopies characterized by different probing depths, namely X-ray magnetic circular dichroism and photoelectron spectroscopy. We thus reveal that the symmetry breaking induced at the Rh-terminated surface stabilizes a surface ferromagnetic layer involving five planes of Fe and Rh atoms in the nominally antiferromagnetic phase at room temperature. First-principles calculations provide a microscopic description of the structural relaxation and the electron spin-density distribution that fully support the experimental findings.",1508.01777v1 2015-09-10,Three-Dimensional Stateful Material Implication Logic,"Monolithic three-dimensional integration of memory and logic circuits could dramatically improve performance and energy efficiency of computing systems. Some conventional and emerging memories are suitable for vertical integration, including highly scalable metal-oxide resistive switching devices (memristors), yet integration of logic circuits proves to be much more challenging. Here we demonstrate memory and logic functionality in a monolithic three-dimensional circuit by adapting recently proposed memristor-based stateful material implication logic. Though such logic has been already implemented with a variety of memory devices, prohibitively large device variability in the most prospective memristor-based circuits has limited experimental demonstrations to simple gates and just a few cycles of operations. By developing a low-temperature, low-variability fabrication process, and modifying the original circuit to increase its robustness to device imperfections, we experimentally show, for the first time, reliable multi-cycle multi-gate material implication logic operation within a three-dimensional stack of monolithically integrated memristors. The direct data manipulation in three dimensions enables extremely compact and high-throughput logic-in-memory computing and, remarkably, presents a viable solution for the Feynman grand challenge of implementing an 8-bit adder at the nanoscale.",1509.02986v1 2018-01-19,"Superconductivity in potassium-doped 2,2$'$-bipyridine","Organic compounds are always promising candidates of superconductors with high transition temperatures. We examine this proposal by choosing 2,2$'$-bipyridine solely composed by C, H, and N atoms. The presence of Meissner effect with a transition temperature of 7.2 K in this material upon potassium doping is demonstrated by the $dc$ magnetic susceptibility measurements. The real part of the $ac$ susceptibility exhibits the same transition temperature as that in $dc$ magnetization, and a sharp peak appeared in the imaginary part indicates the formation of the weakly linked superconducting vortex current. The occurence of superconductivity is further supported by the resistance drop at the transition together with its suppression by the applied magnetic fields. The superconducting phase is identified to be K$_3$-2,2$'$-bipyridine from the analysis of Raman scattering spectra. This work not only opens an encouraging window for finding superconductivity after optoelectronics in 2,2$'$-bipyridine-based materials but also offers an example to realize superconductivity from conducting polymers and their derivatives.",1801.06320v2 2018-05-07,The Role of Grain Boundaries under Long-Time Radiation,"Materials containing a high proportion of grain boundaries offer significant potential for the development of radiation-resistent structural materials. However, a proper understanding of the connection between the radiation-induced microstructural behaviour of grain boundary and its impact at long natural time scales is still missing. In this letter, point defect absorption at interfaces is summarised by a jump Robin-type condition at a coarse-grained level, wherein the role of interface microstructure is effectively taken into account. Then a concise formula linking the sink strength of a polycrystalline aggregate with its grain size is introduced, and is well compared with experimental observation. Based on the derived model, a coarse-grained formulation incorporating the coupled evolution of grain boundaries and point defects is proposed, so as to underpin the study of long-time morphological evolution of grains induced by irradiation. Our simulation results suggest that the presence of point defect sources within a grain further accelerates its shrinking process, and radiation tends to trigger the extension of twin boundary sections.",1805.02360v1 2019-09-19,Low compressible BP$_3$N$_6$,"Using first principles calculation, the structural and mechanical properties of BP$_3$N$_6$ which adopts an orthorhombic structure with space group Pna2$_1$ (no. 33), were determined at three different pressure values (0, 20 and 42.4~GPa). The nine independent elastic constants meet all necessary and sufficient conditions for mechanical stability criteria for an orthorhombic crystal. BP$_3$N$_6$ show strong resistance to volume change hence a potential low compressible material. The Vicker's hardness of BP$_3$N$_6$ was found to range between 49-51~GPa for different external pressures imposed on the crystal. These high values of Vicker's hardness implies that BP$_3$N$_6$ is a potential superhard material.",1909.08879v2 2014-08-06,Crystal structure and electronic structure of CePt2In7,"We report a corrected crystal structure for the CePt2In7 superconductor, refined from single crystal x-ray diffraction data. The corrected crystal structure shows a different Pt-In stacking along the c-direction in this layered material than was previously reported. In addition, all the atomic sites are fully occupied with no evidence of atom site mixing, resolving a discrepancy between the observed high resistivity ratio of the material and the atomic disorder present in the previous structural model The Ce-Pt distance and coordination is typical of that seen in all other reported Ce_nM_mIn_3n+2m compounds. Our band structure calculations based on the correct structure reveal three bands at the Fermi level that are more three dimensional than those previously proposed, and Density functional theory (DFT) calculations show that the new structure has a significantly lower energy.",1408.1246v1 2017-01-30,Pressure-induced superconductivity and topological quantum phase transitions in a quasi-one-dimensional topological insulator: Bi4I4,"Superconductivity and topological quantum states are two frontier fields of research in modern condensed matter physics. The realization of superconductivity in topological materials is highly desired, however, superconductivity in such materials is typically limited to two- or three-dimensional materials and is far from being thoroughly investigated. In this work, we boost the electronic properties of the quasi-one-dimensional topological insulator bismuth iodide \b{eta}-Bi4I4 by applying high pressure. Superconductivity is observed in \b{eta}-Bi4I4 for pressures where the temperature dependence of the resistivity changes from a semiconducting-like behavior to that of a normal metal. The superconducting transition temperature Tc increases with applied pressure and reaches a maximum value of 6 K at 23 GPa, followed by a slow decrease. Our theoretical calculations suggest the presence of multiple pressure-induced topological quantum phase transitions as well as a structural-electronic instability.",1701.08860v1 2019-03-12,Structural and electronic properties of the spin-filter material CrVTiAl with disorder,"The effects of chemical disorder on the transport properties of the spin-filter material CrVTiAl are investigated experimentally and theoretically. Synchrotron X-ray diffraction experiments on bulk CrVTiAl and the associated Rietveld analysis indicate that the crystal structure consists primarily of a mixture of a partially ordered B2 phase, a fully disordered A2 phase and a small component of an ordered L2\textsubscript{1} or Y phase. High temperature resistivity measurements confirm the existence of a band gap. First-principles, all-electron, self-consistent electronic structure computations show that the chemically disordered A2 and B2 phases are metallic, while the spin-filter properties of the ideal Y-type phase are preserved in the presence of L2\textsubscript{1} disorder. The Hall coefficient is found to decrease with increasing temperature, similar to the measured increase in the conductivity, indicating the presence of thermally activated semiconductor-like carriers.",1903.05004v1 2019-01-28,Effect of Bi Substitution on Thermoelectric Properties of SbSe2-based Layered Compounds NdO$_{0.8}$F$_{0.2}$Sb$_{1-x}$Bi$_x$Se$_2$,"Although SbSe2-based layered compounds have been predicted to be high-performance thermoelectric materials and topological materials, most of these compounds obtained experimentally have been insulators so far. Here, we present the effect of Bi substitution on the thermoelectric properties of SbSe2-based layered compounds NdO0.8F0.2Sb1-xBixSe2 (x = 0-0.4). The room temperature electrical resistivity is decreased to 8.0 * 10^-5 ohmm for x = 0.4. The electrical power factor is calculated to be 1.4 * 10^-4 W/mK^2 at 660 K, which is in reasonable agreement with combined Jonker and Ioffe analysis. The room-temperature lattice thermal conductivity of less than 1 W/mK is almost independent of x, in contrast to the point-defect scattering model for conventional alloys. The present work provides an avenue for exploring SbSe2-based insulating and BiSe2-based conducting systems.",1901.09909v1 2020-08-21,An unexplored MBE growth mode reveals new properties of superconducting NbN,"Accessing unexplored conditions in crystal growth often reveals remarkable surprises and new regimes of physical behavior. In this work, performing molecular beam epitaxy of the technologically important superconductor NbN at temperatures greater than 1000$^\circ$C, higher than in the past, is found to reveal persistent RHEED oscillations throughout the growth, atomically smooth surfaces, normal metal resistivities as low as 37$\mu\Omega$-cm and superconducting critical temperatures in excess of 15 K. Most remarkably, a reversal of the sign of the Hall coefficient is observed as the NbN films are cooled, and the high material quality allows the first imaging of Abrikosov vortex lattices in this superconductor.",2008.09596v3 2020-09-25,A Possible Method of Carbon Deposit Mapping on Plasma Facing Components Using Infrared Thermography,"The material eroded from the surface of plasma facing components is redeposited partly close to high heat flux areas. At these locations, the deposit is heated by the plasma and the deposition pattern evolves depending on the operation parameters. The mapping of the deposit is still a matter of intense scientific activity, especially during the course of experimental campaigns. A method based on the comparison of surface temperature maps, obtained in situ by infrared cameras and by theoretical modelling is proposed. The difference between the two is attributed to the thermal resistance added by deposited material, and expressed as a deposit thickness. The method benefits of elaborated imaging techniques such as possibility theory and fuzzy logics. The results are consistent with deposit maps obtained by visual inspection during shutdowns.",2010.06374v1 2020-10-29,Nature of native atomic defects in ZrTe$_5$ and their impact on the low-energy electronic structure,"Over the past decades, investigations of the anomalous low-energy electronic properties of ZrTe$_5$ have reached a wide array of conclusions. An open question is the growth method's impact on the stoichiometry of ZrTe$_5$ samples, especially given the very small density of states near its chemical potential. Here we report on high resolution scanning tunneling microscopy and spectroscopy measurements performed on samples grown via different methods. Using density functional theory calculations, we identify the most prevalent types of atomic defects on the surface of ZrTe$_5$, namely Te vacancies and intercalated Zr atoms. Finally, we precisely quantify their density and outline their role as ionized defects in the anomalous resistivity of this material.",2010.15513v1 2021-11-17,Anisotropic superconductivity and unusually robust electronic critical field in single crystal La$_{7}$Ir$_{3}$,"Polycrystalline La$_{7}$Ir$_{3}$ is reported to show superconductivity breaking time-reversal symmetry while also having an isotropic $s$-wave gap. Single crystals of this noncentrosymmetric superconductor are highly desirable to understand the nature of the electron pairing mechanism in this system. Here we report the growth of high-quality single crystals of La$_{7}$Ir$_{3}$ by the Czochralski method. The structural and superconducting properties of these large crystals have been investigated using x-rays, magnetization, resistivity and heat capacity measurements. We observe a clear anisotropy in the lower and upper critical fields for magnetic fields applied parallel and perpendicular to the hexagonal $c$ axis. We also report the presence of a robust electronic critical field, that diverges from the upper critical field derived from heat capacity, which is the hallmark of surface superconductivity.",2111.09239v2 2022-01-09,Phase field fracture predictions of microscopic bridging behaviour of composite materials,"We investigate the role of microstructural bridging on the fracture toughness of composite materials. To achieve this, a new computational framework is presented that integrates phase field fracture and cohesive zone models to simulate fibre breakage, matrix cracking and fibre-matrix debonding. The composite microstructure is represented by an embedded cell at the vicinity of the crack tip, whilst the rest of the sample is modelled as an anisotropic elastic solid. The model is first validated against experimental data of transverse matrix cracking from single-notched three-point bending tests. Then, the model is extended to predict the influence of grain bridging, brick-and-mortar microstructure and 3D fibre bridging on crack growth resistance. The results show that these microstructures are very efficient in enhancing the fracture toughness via fibre-matrix debonding, fibre breakage and crack deflection. In particular, the 3D fibre bridging effect can increase the energy dissipated at failure by more than three orders of magnitude, relative to that of the bulk matrix; well in excess of the predictions obtained from the rule of mixtures. These results shed light on microscopic bridging mechanisms and provide a virtual tool for developing high fracture toughness composites.",2201.03066v1 2022-10-30,Linear nonsaturating magnetoresistance in kagome superconductor CsV3Sb5 thin flakes,"Linear nonsaturating magnetoresistance (LMR) represents a class of anomalous resistivity response to external magnetic field that has been observed in a variety of materials including but not limited to topological semi-metals, high-Tc superconductors and materials with charge/spin density wave (CDW/SDW) orders. Here we report the observation of LMR in layered kagome superconductor and CDW material CsV3Sb5 thin flakes, as well as the dimensional crossover and temperature (T) crossover of such LMR. Specifically, in ultrathin CsV3Sb5 crystals, the magnetoresistance (MR) exhibits a crossover from LMR at low T to quadratic B dependence above the CDW transition temperature; the MR also exhibits a crossover from LMR to sublinear MR for sample thickness at around ~20 nm at low T. We discuss several possible origins of the LMR and attribute the effect to two-dimensional (2D) CDW fluctuations. Our results may provide a new perspective for understanding the interactions between competing orders in kagome superconductors.",2210.16890v1 2023-08-09,Superionic phase transition of copper(I) sulfide and its implication for purported superconductivity of LK-99,"Lee, Kim, and coworkers have recently claimed room-temperature and ambient-pressure superconductivity in a copper-doped lead apatite material named LK-99. However, the polycrystalline material synthesized has a significant fraction of copper(I) sulfide. Copper(I) sulfide has a known phase transition at 104 degrees C from an ordered low-temperature phase to a high-temperature superionic phase. As a result of this phase transition, copper(I) sulfide exhibits sharp transitions in electrical resistivity and heat capacity, which are expected to coincide with the temperature-induced transitions reported for LK-99. This implies that LK-99 must be synthesized without any copper(I) sulfide to allow unambiguous validation of the superconducting properties of LK-99.",2308.05222v3 2023-11-15,Strongly pinned skyrmionic bubbles and higher-order nonlinear Hall resistances at the interface of Pt/FeSi bilayer,"Engineering of magnetic heterostructures for spintronic applications has entered a new phase, driven by the recent discoveries of topological materials and exfoliated van der Waals materials. Their low-dimensional properties can be dramatically modulated in designer heterostructures via proximity effects from adjacent materials, thus enabling the realization of diverse quantum states and functionalities. Here we investigate spin-orbit coupling (SOC) proximity effects of Pt on the recently discovered quasi-two-dimensional ferromagnetic state at FeSi surface. Skyrmionic bubbles (SkBs) are formed as a result of the enhanced interfacial Dzyloshinskii-Moriya interaction. The strong pinning effects on the SkBs are evidenced from the significant dispersion in size and shape of the SkBs and are further identified as a greatly enhanced threshold current density required for depinning of the SkBs. The robust integrity of the SkB assembly leads to the emergence of higher-order nonlinear Hall effects in the high current density regime, which originate from nontrivial Hall effects due to the noncollinearity of the spin texture, as well as from the current-induced magnetization dynamics via the augmented spin-orbit torque.",2311.08730v1 2023-11-21,Reliable lift-off patterning of graphene dispersions for humidity sensors,"Dispersion-based graphene materials are promising candidates for various sensing applications. They offer the advantage of relatively simple and fast deposition via spin-coating, Langmuir-Blodgett deposition, or inkjet printing. Film uniformity and reproducibility remain challenging in all of these deposition methods. Here, we demonstrate, characterize, and successfully apply a scalable structuring method for graphene dispersions. The method is based on a standard lift-off process, is simple to implement, and increases the film uniformity of graphene devices. It is also compatible with standard semiconductor manufacturing methods. We investigate two different graphene dispersions via Raman spectroscopy and Atomic Force Microscopy and observe no degradation of the material properties by the structuring process. Furthermore, we achieve high uniformity of the structured patterns and homogeneous graphene flake distribution. Electrical characterizations show reproducible sheet resistance values correlating with material quantity and uniformity. Finally, repeatable humidity sensing is demonstrated with van der Pauw devices, with sensing limits of less than 1% relative humidity.",2311.12650v2 2024-04-10,Optimal Matching of Thermal Vibrations into Carbon Nanotubes,"Carbon nanotubes (CNTs) are promising candidates to improve the thermal conductivity of nano-composites. The main obstacle to these applications is the extremely high thermal boundary (Kapitza) resistance between the CNTs and their matrix. In this theoretical work our goal is to maximize the heat flux through the CNT by functionalizing the CNT ends. We use a Landauer approach to calculate and optimize the energy flux from a soft to a hard material in one dimension through a connecting continuous medium of varying elasticity and density. The transmission probability of phonons through the system is calculated both numerically and analytically. We find that over 90% of the maximum heat flux into CNT is possible for 1nm length of the intermediate material at room temperature (300K).",2404.06938v1 2010-11-12,Suspension and Measurement of Graphene and Bi2Se3 Atomic Membranes,"Coupling high quality, suspended atomic membranes to specialized electrodes enables investigation of many novel phenomena, such as spin or Cooper pair transport in these two dimensional systems. However, many electrode materials are not stable in acids that are used to dissolve underlying substrates. Here we present a versatile and powerful multi-level lithographical technique to suspend atomic membranes, which can be applied to the vast majority of substrate, membrane and electrode materials. Using this technique, we fabricated suspended graphene devices with Al electrodes and mobility of 5500 cm^2/Vs. We also demonstrate, for the first time, fabrication and measurement of a free-standing thin Bi2Se3 membrane, which has low contact resistance to electrodes and a mobility of >~500 cm^2/Vs.",1011.2837v1 2011-11-04,Dual-gated bilayer graphene hot electron bolometer,"Detection of infrared light is central to diverse applications in security, medicine, astronomy, materials science, and biology. Often different materials and detection mechanisms are employed to optimize performance in different spectral ranges. Graphene is a unique material with strong, nearly frequency-independent light-matter interaction from far infrared to ultraviolet, with potential for broadband photonics applications. Moreover, graphene's small electron-phonon coupling suggests that hot-electron effects may be exploited at relatively high temperatures for fast and highly sensitive detectors in which light energy heats only the small-specific-heat electronic system. Here we demonstrate such a hot-electron bolometer using bilayer graphene that is dual-gated to create a tunable bandgap and electron-temperature-dependent conductivity. The measured large electron-phonon heat resistance is in good agreement with theoretical estimates in magnitude and temperature dependence, and enables our graphene bolometer operating at a temperature of 5 K to have a low noise equivalent power (33 fW/Hz1/2). We employ a pump-probe technique to directly measure the intrinsic speed of our device, >1 GHz at 10 K.",1111.1202v1 2012-11-08,Structural phase transformations in metallic grain boundaries,"Structural transformations at interfaces are of profound fundamental interest as complex examples of phase transitions in low-dimensional systems. Despite decades of extensive research, no compelling evidence exists for structural transformations in high-angle grain boundaries in elemental systems. Here we show that the critical impediment to observations of such phase transformations in atomistic modeling has been rooted in inadequate simulation methodology. The proposed new methodology allows variations in atomic density inside the grain boundary and reveals multiple grain boundary phases with different atomic structures. Reversible first-order transformations between such phases are observed by varying temperature or injecting point defects into the boundary region. Due to the presence of multiple metastable phases, grain boundaries can absorb significant amounts of point defects created inside the material by processes such as irradiation. We propose a novel mechanism of radiation damage healing in metals which may guide further improvements in radiation resistance of metallic materials through grain boundary engineering.",1211.1756v2 2014-10-10,Topological Origin of Fracture Toughening in Complex Solids: the Viewpoint of Rigidity Theory,"In order to design tougher materials, it is crucial to understand the relationship between their composition and their resistance to fracture. To this end, we investigate the fracture toughness of usual sodium silicate glasses (NS) and complex calcium--silicate--hydrates (CSH), the binding phase of cement. Their atomistic structure is described in the framework of the topological constraints theory, or rigidity theory. We report an analogous rigidity transition, driven by pressure in NS and by composition in CSH. Relying both on simulated and available experimental results, we show that optimally constrained isostatic systems show improved fracture toughness. The flexible to stressed--rigid transition is shown to be correlated to a ductile-to-brittle transition, with a local minimum of the brittleness for isostatic system. This fracture toughening arises from a reversible molecular network, allowing optimal stress relaxation and crack blunting behaviors. This opens the way to the discovery of high-performance materials, designed at the molecular scale.",1410.2916v1 2015-02-09,Pressure-induced superconductivity in the three-dimensional Dirac semimetal Cd3As2,"The recently discovered Dirac and Weyl semimetals are new members of topological materials. Starting from them, topological superconductivity may be achieved, e.g. by carrier doping or applying pressure. Here we report high-pressure resistance and X-ray diffraction study of the three-dimensional topological Dirac semimetal Cd3As2. Superconductivity with Tc ~ 2.0 K is observed at 8.5 GPa. The Tc keeps increasing to about 4.0 K at 21.3 GPa, then shows a nearly constant pressure dependence up to the highest pressure 50.9 GPa. The X-ray diffraction measurements reveal a structure phase transition around 3.5 GPa. Our observation of superconductivity in pressurized topological Dirac semimetal Cd3As2 provides a new candidate for topological superconductor, as argued in a recent point contact study and a theoretical work.",1502.02509v2 2017-06-19,Electrical and Thermal Transport at the Planckian Bound of Dissipation in the Hydrodynamic Electron Fluid of WP2,"Materials with strongly-correlated electrons exhibit interesting phenomena such as metal-insulator transitions and high-temperature superconductivity. In stark contrast to ordinary metals, electron transport in these materials is thought to resemble the flow of viscous fluids. Despite their differences, it is predicted that transport in both, conventional and correlated materials, is fundamentally limited by the uncertainty principle applied to energy dissipation. Here we discover hydrodynamic electron flow in the Weyl-semimetal tungsten phosphide (WP2). Using thermal and magneto-electric transport experiments, we observe the transition from a conventional metallic state, at higher temperatures, to a hydrodynamic electron fluid below 20 K. The hydrodynamic regime is characterized by a viscosity-induced dependence of the electrical resistivity on the square of the channel width, and by the observation of a strong violation of the Wiedemann-Franz law. From magneto-hydrodynamic experiments and complementary Hall measurements, the relaxation times for momentum and thermal energy dissipating processes are extracted. Following the uncertainty principle, both are limited by the Planckian bound of dissipation, independent of the underlying transport regime.",1706.05925v2 2017-09-22,On Extracting Mechanical Properties from Nanoindentation at Temperatures up to 1000$^{\circ}$C,"Alloyed MCrAlY bond coats, where M is usually cobalt and/or nickel, are essential parts of modern turbine blades, imparting environmental resistance while mediating thermal expansivity differences. Nanoindentation allows the determination of their properties without the complexities of traditional mechanical tests, but was not previously possible near turbine operating temperatures. Here, we determine the hardness and modulus of CMSX-4 and an Amdry-386 bond coat by nanoindentation up to 1000$^{\circ}$C. Both materials exhibit a constant hardness until 400$^{\circ}$C followed by considerable softening, which in CMSX-4 is attributed to the multiple slip systems operating underneath a Berkovich indenter. The creep behaviour has been investigated via the nanoindentation hold segments. Above 700$^{\circ}$C, the observed creep exponents match the temperature-dependence of literature values in CMSX-4. In Amdry-386, nanoindentation produces creep exponents very close to literature data, implying high-temperature nanoindentation may be powerful in characterising these coatings and providing inputs for material, model and process optimisations.",1709.07714v1 2017-03-16,Equivalence of Effective Medium and Random Resistor Network models for disorder-induced unsaturating linear magnetoresistance,"A linear unsaturating magnetoresistance at high perpendicular magnetic fields, together with a quadratic positive magnetoresistance at low fields, has been seen in many different experimental materials, ranging from silver chalcogenides and thin films of InSb to topological materials like graphene and Dirac semimetals. In the literature, two very different theoretical approaches have been used to explain this classical magnetoresistance as a consequence of sample disorder. The phenomenological Random Resistor Network model constructs a grid of four-terminal resistors, each with a varying random resistance. The Effective Medium Theory model imagines a smoothly varying disorder potential that causes a continuous variation of the local conductivity. Here, we demonstrate numerically that both models belong to the same universality class and that a restricted class of the Random Resistor Network is actually equivalent to the Effective Medium Theory. Both models are also in good agreement with experiments on a diverse range of materials. Moreover, we show that in both cases, a single parameter, i.e. the ratio of the fluctuations in the carrier density to the average carrier density, completely determines the magnetoresistance profile.",1703.05478v1 2017-08-24,Probing the Fermi surface and magnetotransport properties in MoAs$_{2}$,"Transition metal dipnictides (TMDs) have recently been identified as possible candidates to host topology protected electronic band structure. These materials belong to an isostructural family and show several exotic transport properties. Especially, the large values of magnetoresistance (MR) and carrier mobility have drawn significant attention from the perspective of technological applications. In this report, we have investigated the magnetotransport and Fermi surface properties of single crystalline MoAs$_{2}$, another member of this group of compounds. Field induced resistivity plateau and a large MR have been observed, which are comparable to several topological systems. Interestingly, in contrast to other isostructural materials, the carrier density in MoAs$_{2}$ is quite high and shows single-band dominated transport. The Fermi pockets, which have been identified from the quantum oscillation, are largest among the members of this group and have significant anisotropy with crystallographic direction. Our first-principles calculations reveal a substantial difference between the band structures of MoAs$_{2}$ and other TMDs. The calculated Fermi surface consists of one electron pocket and another 'open-orbit' hole pocket, which has not been observed in TMDs so far.",1708.07294v1 2019-03-18,Zirconia UV-curable colloids for additive manufacturing via hybrid inkjet printing-stereolithography,"Currently, additive manufacturing of ceramics by stereolithography (SLA) is limited to single materials and by a poor thickness resolution that strongly depends on the ceramic particles-UV light interaction. Combining selective laser curing with inkjet printing represents a novel strategy to overcome these constrains. Nonetheless, this approach requires UV-curable inks that allow hardening of the printed material and sintering to high density. In this work, we report how to design an ink for inkjet printing of yttria stabilized zirconia (YSZ) which can be impressed by addition of UV-curable monomers. We especially show how the formulation of the inks and particularly the UV-monomer concentration impacts the printability and the UV-curing. This leads to prints that are resistant to solvent washing first and densify to 96% dense YSZ layers after sintering.",1903.07731v1 2019-12-23,Large $d_{33}$ Piezoelectric-Polymer Composites For RF Acoustic Resonators,"While piezoelectric transduction enables designing acoustic resonators operating at multi-GHz frequencies, the deposition of piezoelectric materials typically requires high temperature processes and specific crystallographic orientation of substrates, thus imposing a limitation on materials that could be used. In this paper we present a piezoelectrically transduced thickness mode acoustic resonator that employs piezoelectric (PMNPT) nanoparticles embedded in a polymer (SU8) matrix. This composite material is deposited using standard resist-spin coaters and is thus compatible with a variety of substrates. The device presented here uses a double side polished single crystal silicon wafer as the low loss acoustic substrate for the resonator and $1.7\mu m$ thick SU8-PMNPT composite film as the actuator, and exhibits large effective piezoelectric coefficient $(d_{33})$ of $216pm/V$, and we experimentally demonstrate efficient transduction of acoustic resonances at frequencies up to $1.5GHz$.",1912.10713v1 2021-01-25,Polycaprolactone/graphite nanoplates composite nanopapers,"Nanopapers based on graphene and related materials were recently proposed for application in heat spreader applications. To overcome typical limitations in brittleness of such materials, this work addressed the combination of graphite nanoplatelets (GNP) with a soft, tough and crystalline polymer, acting as an efficient binder between nanoplates. With this aim, polycaprolactone (PCL) was selected and exploited in this paper. The crystalline organization of PCL within the nanopaper was studied to investigate the effect of polymer confinement between GNP. Thermomechanical properties were studied by dynamic mechanical analyses at variable temperature and creep measurements at high temperature, demonstrating superior resistance at temperatures well above PCL melting. Finally, the heat conduction properties on the nanopapers were evaluated, resulting in outstanding values above 150 Wm-1K-1.",2101.10283v1 2019-11-13,Portable and wireless signal transducer for field testing of environmental sensors based on 2D materials,"In this paper we present the design and fabrication of a portable device for environmental monitoring applications. This novel hand-held apparatus monitors the changes in the resistance of a sensing surface with a high accuracy and resolution and transmits the recorded data wirelessly to a cellphone. Such a design offers a solution for field testing of environmental sensors. The tested sensing surface in this study is based on an ultrathin material: graphene, which is placed on the surface of a Si/SiO2 wafer. This signal transducer and wireless communication system form together an ideal platform to harvest the sensitivity and selectivity of 2D materials for gas sensing applications.",1911.05764v2 2022-01-08,Dynamical Mean Field Studies of Infinite Layer Nickelates: Physics Results and Methodological Implications,"This article summarizes recent work on the many-body (beyond density functional theory) electronic structure of layered rare-earth nickelates, both in the context of the materials themselves and in comparison to the high-temperature superconducting (high-$T_c$) layered copper-oxide compounds. It aims to outline the current state of our understanding of layered nickelates and to show how the analysis of these fascinating materials can shed light on fundamental questions in modern electronic structure theory. A prime focus is determining how the interacting physics defined over a wide energy range can be estimated and ""downfolded"" into a low energy theory that would describe the relevant degrees of freedom on the $\sim 0.5$ eV scale and that could be solved to determine superconducting and spin and charge density wave phase boundaries, temperature-dependent resistivities, and dynamical susceptibilities.",2201.02852v1 2022-03-04,Broadband Cross-Circular Polarization Carpet Cloaking based on a Phase Change Material Metasurface in the Mid-infrared Region,"In view of the fact that most invisibility devices focus on linear polarization cloaking and that the characteristics of mid infrared cloaking are rarely studied, we propose a cross circularly polarized invisibility carpet cloaking device in the mid infrared band. Based on the Pancharatnam Berry phase principle, the unit cells with the cross circular polarization gradient phase were carefully designed and constructed into a metasurface. In order to achieve tunable cross circular polarization carpet cloaks, a phase change material is introduced into the design of the unit structure. When the phase change material is in amorphous and crystalline states, the proposed metasurface unit cells can achieve high efficiency cross polarization conversion and reflection intensity can be tuned. According to the phase compensation principle of carpet cloaking, we construct a metasurface cloaking device with a phase gradient using the designed unit structure. From the near and far field distributions, the cross circular polarization cloaking property is confirmed in the broadband wavelength range. The proposed cloaking device can effectively resist detection of cross-circular polarization.",2203.02222v1 2022-03-06,Scaled indium oxide transistors fabricated using atomic layer deposition,"In order to continue to improve integrated circuit performance and functionality, scaled transistors with short channel lengths and low thickness are needed. But the further scaling of silicon-based devices and the development of alternative semiconductor channel materials that are compatible with current fabrication processes is challenging. Here we report atomic-layer-deposited indium oxide transistors with channel lengths down to 8 nm, channel thicknesses down to 0.5 nm and equivalent dielectric oxide thickness down to 0.84 nm. Due to the scaled device dimensions and low contact resistance, the devices exhibit high on-state currents of 3.1 A/mm at a drain voltage of 0.5 V and a transconductance of 1.5 S/mm at a drain voltage 1 V. Our devices are a promising alternative channel material for scaled transistors with back-end-of-line processing compatibility.",2203.02869v1 2022-10-18,Nanoscale friction controlled by top layer thickness in [LaMnO$_{3}$]$_{m}$/[SrMnO$_{3}$]$_{n}$ superlattices,"We conducted lateral force microscopy measurements on seven [LaMnO$_{3}$]$_{m}$/[SrMnO$_{3}$]$_{n}$ superlattices with varied layer thicknesses. We observe that the friction forces and the friction coefficients initially increase with increasing LaMnO3 top layer thickness, followed by saturation when the top layer thickness exceeds a few nanometers. These observations clearly demonstrate that sliding friction is affected by sub-surface material properties to a depth of several nanometers and is not just determined by dynamics in the contact interface. We argue that the sub-surface dissipated energy is governed by damping in the elastically strained volume below the AFM tip, an effect which we estimate via thermoelasticity. The absence of a correlation between friction and the thermal resistivity of our superlattices shows furthermore that high-frequency phonons and heat conduction do not play a role in determining friction. Our observations thus demonstrate that friction can be tailored by sub-surface material properties.",2210.09677v1 2023-05-15,Superconductivity at epitaxial LaTiO3-KTaO3 interfaces,"Design of epitaxial interfaces is a pivotal way to engineer artificial structures where new electronic phases can emerge. Here we report a systematic emergence of interfacial superconducting state in epitaxial heterostructures of LaTiO3 and KTaO3. The superconductivity transition temperature increases with decreasing the thickness of LaTiO3. Such behavior is observed for both (110) and (111) crystal oriented structures. For thick samples, the finite resistance developing below the superconducting transition temperature increases with increasing LaTiO3 thickness. Consistent with previous reports, the (001) oriented heterointerface features high electron mobility of 250 cm2/Vs and shows no superconducting transition down to 40 mK. Our results imply a non-trivial impact of LaTiO3 on the superconducting state and indicate how superconducting KTaO3 interfaces can be integrated with other oxide materials.",2305.08304v1 2024-02-16,Erosion Study of Tungsten Carbide films under 100 keV Kr+ ion irradiation,"Tungsten carbide (WC) stands out as a crucial material for exploration in extreme environments due to its resistance to radiation and impressive mechanical strength. Widely utilized in cutting tools, high-wear components, and as a potential contender for plasma-facing material in nuclear reactors, WC's erosion behavior under surrogate irradiations is a subject of investigation. In the present work, WC films were synthesized at two different substrate temperatures of 400 K and 600 K using RF sputtering and were then irradiated with 100 keV Kr1+ ions at a fluence of 1x1017 ions/cm2. The crystalline phases of as deposited WC films were confirmed by glancing incidence X-ray diffraction (GIXRD) measurements. Rutherford Backscattering Spectrometry (RBS) was employed to determine the thicknesses of pristine samples and the sputtering rate by measuring the difference in the areal densities of the pristine and irradiated films. The erosion rate of both types of films was found to be ~ 1.6 atoms per incident Kr+ ion. These findings contribute to a foundational comprehension of the radiation tolerance behavior of WC thin films, crucial for their performance in the demanding conditions of extreme radiation.",2402.10461v1 2001-05-22,Infrared optical properties of Pr2CuO4,"The ab-plane reflectance of a Pr2CuO4 single crystal has been measured over a wide frequency range at a variety of temperatures, and the optical properties determined from a Kramers-Kronig analysis. Above ~ 250 K, the low frequency conductivity increases quickly with temperature; the resistivity follows the form e^(E_a/k_BT), where E_a ~ 0.17 eV is much less than the inferred optical gap of ~ 1.2 eV. Transport measurements show that at low temperature the resistivity deviates from activated behavior and follows the form e^[(T_0/T)^1/4], indicating that the dc transport in this material is due to variable-range hopping between localized states in the gap. The four infrared-active Eu modes dominate the infrared optical properties. Below ~ 200 K, a striking new feature appears near the low-frequency Eu mode, and there is additional new fine structure at high frequency. A normal coordinate analysis has been performed and the detailed nature of the zone-center vibrations determined. Only the low-frequency Eu mode has a significant Pr-Cu interaction. Several possible mechanisms related to the antiferromagnetism in this material are proposed to explain the sudden appearance of this and other new spectral features at low temperature.",0105445v2 2006-11-29,What is the valence of a correlated solid? The double life of delta-plutonium,"Plutonium displays phase transitions with enormous volume differences among its phases and both its Pauli like magnetic susceptibility and resistivity are an order of magnitude larger than those of simple metals. Curium is also highly resistive but its susceptibility is Curie-like at high temperatures and orders antiferromagnetically at low temperatures. The anomalous properties of the late actinides stem from the competition between the itinerancy and localization of its f electrons, which makes the late actinides elemental strongly correlated materials. A central problem in this field is to understand the mechanism by which these materials resolve these conflicting tendencies. In this letter we identify the electronic mechanisms responsible for the anomalous behaviour of late actinides. We revisit the concept of valence using theoretical approach that treats magnetism, Kondo screening, atomic multiplet effects, spin orbit coupling and crystal field splitting on the same footing. Plutonium is found to be in a rare mixed valent state, namely its ground state is a superposition of two distinct valencies. Curium settles in a single valence magnetically ordered state at low temperatures. The f7 atomic configuration of Curium is contrasted with the multiple configuration manifolds present in Plutonium ground state which we characterize by a valence histogram. The balance between the Kondo screening and magnetism is determined by the competition between spin orbit coupling and the strength of atomic multiplets which is in turn regulated by the degree of itinerancy. The approach presented here, highlights the electronic origin of the bonding anomalies in plutonium and can be applied to predict generalized valences and the presence or absence of magnetism in other compounds starting from first principles.",0611760v1 2009-05-08,Magnetotransport in polycrystalline La$_{2/3}$Sr$_{1/3}$MnO$_{3}$ thin films of controlled granularity,"Polycrystalline La$_{2/3}$Sr$_{1/3}$MnO$_{3}$ (LSMO) thin films were synthesized by pulsed laser ablation on single crystal (100) yttria-stabilized zirconia (YSZ) substrates to investigate the mechanism of magneto-transport in a granular manganite. Different degrees of granularity is achieved by using the deposition temperature (T$_{D}$) of 700 and 800 $^{0}$C. Although no significant change in magnetic order temperature (T$_C$) and saturation magnetization is seen for these two types of films, the temperature and magnetic field dependence of their resistivity ($\rho$(T, H)) is strikingly dissimilar. While the $\rho$(T,H) of the 800 $^{0}$C film is comparable to that of epitaxial samples, the lower growth temperature leads to a material which undergoes insulator-to-metal transition at a temperature (T$_{P}$ $\approx$ 170 K) much lower than T$_C$. At T $\ll$ T$_P$, the resistivity is characterized by a minimum followed by ln $\emph{T}$ divergence at still lower temperatures. The high negative magnetoresistance ($\approx$ 20$%$) and ln $\emph{T}$ dependence below the minimum are explained on the basis of Kondo-type scattering from blocked Mn-spins in the intergranular material. Further, a striking feature of the T$_D$ = 700 $^{0}$C film is its two orders of magnitude larger anisotropic magnetoresistance (AMR) as compared to the AMR of epitaxial films. We attribute it to unquenching of the orbital angular momentum of 3d electrons of Mn ions in the intergranular region where crystal field is poorly defined.",0905.1306v1 2009-12-27,Topological Insulator Nanowires and Nanoribbons,"Recent theoretical calculations and photoemission spectroscopy measurements on the bulk Bi2Se3 material show that it is a three-dimensional topological insulator possessing conductive surface states with nondegenerate spins, attractive for dissipationless electronics and spintronics applications. Nanoscale topological insulator materials have a large surface-to-volume ratio that can manifest the conductive surface states and are promising candidates for devices. Here we report the synthesis and characterization of high quality single crystalline Bi2Se3 nanomaterials with a variety of morphologies. The synthesis of Bi2Se3 nanowires and nanoribbons employs Au-catalyzed vapor-liquid-solid (VLS) mechanism. Nanowires, which exhibit rough surfaces, are formed by stacking nanoplatelets along the axial direction of the wires. Nanoribbons are grown along [11-20] direction with a rectangular cross-section and have diverse morphologies, including quasi-one-dimensional, sheetlike, zigzag and sawtooth shapes. Scanning tunneling microscopy (STM) studies on nanoribbons show atomically smooth surfaces with ~ 1 nm step edges, indicating single Se-Bi-Se-Bi-Se quintuple layers. STM measurements reveal a honeycomb atomic lattice, suggesting that the STM tip couples not only to the top Se atomic layer, but also to the Bi atomic layer underneath, which opens up the possibility to investigate the contribution of different atomic orbitals to the topological surface states. Transport measurements of a single nanoribbon device (four terminal resistance and Hall resistance) show great promise for nanoribbons as candidates to study topological surface states.",0912.5045v1 2010-06-02,Antiferromagnetic Mott insulating state in single crystals of the hexagonal lattice material Na2IrO3,"We have synthesized single crystals of Na_2IrO_3 and studied their structure, transport, magnetic, and thermal properties using powder x-ray diffraction (PXRD), electrical resistivity, isothermal magnetization M versus magnetic field H, magnetic susceptibility \chi versus temperature T, and heat capacity C versus T measurements. Na_2IrO_3 crystallizes in the monoclinic \emph{C2/c} (No. 15) type structure which is made up of Na and NaIr_2O_6 layers alternately stacked along the c axis. The \chi(T) data show Curie-Weiss behavior at high T > 200K with an effective moment \mu_eff = 1.82(1) \mu_B indicating an effective spin S_eff = 1/2 on the Ir^4+ moments. A large Weiss temperature \theta = - 116(3)K indicates substantial antiferromagnetic interactions between these S_eff = 1/2, Ir^4+ moments. Sharp anomalies in \chi(T) and C(T) data indicate that Na_2IrO_3 undergoes a transition into a long-range antiferromagnetically ordered state below T_N = 15 K. The magnetic entropy at T_N is only about 20% of what is expected for S_eff = 1/2 moment ordering. The reduced entropy and the small ratio T_N/\theta \approx 0.13 suggest geometrical magnetic frustration and/or low-dimensional magnetic interactions in Na_2IrO_3. In plane resistivity measurements show insulating behavior. This together with the local moment magnetism indicates that bulk Na_2IrO_3 is a Mott insulator.",1006.0437v1 2010-11-02,Graphene: from materials science to particle physics,"Since its discovery in 2004, graphene, a two-dimensional hexagonal carbon allotrope, has generated great interest and spurred research activity from materials science to particle physics and vice versa. In particular, graphene has been found to exhibit outstanding electronic and mechanical properties, as well as an unusual low-energy spectrum of Dirac quasiparticles giving rise to a fractional quantum Hall effect when freely suspended and immersed in a magnetic field. One of the most intriguing puzzles of graphene involves the low-temperature conductivity at zero density, a central issue in the design of graphene-based nanoelectronic components. While suspended graphene experiments have shown a trend reminiscent of semiconductors, with rising resistivity at low temperatures, most theories predict a constant or even decreasing resistivity. However, lattice field theory calculations have revealed that suspended graphene is at or near the critical coupling for excitonic gap formation due to strong Coulomb interactions, which suggests a simple and straightforward explanation for the experimental data. In this contribution we review the current status of the field with emphasis on the issue of gap formation, and outline recent progress and future points of contact between condensed matter physics and Lattice QCD.",1011.0643v1 2013-03-04,Statistical Study of Deep Sub-Micron Dual-Gated Field-Effect Transistors on Monolayer CVD Molybdenum Disulfide Films,"Monolayer Molybdenum Disulfide (MoS2) with a direct band gap of 1.8 eV is a promising two-dimensional material with a potential to surpass graphene in next generation nanoelectronic applications. In this letter, we synthesize monolayer MoS2 on Si/SiO2 substrate via chemical vapor deposition (CVD) method and comprehensively study the device performance based on dual-gated MoS2 field-effect transistors. Over 100 devices are studied to obtain a statistical description of device performance in CVD MoS2. We examine and scale down the channel length of the transistors to 100 nm and achieve record high drain current of 62.5 mA/mm in CVD monolayer MoS2 film ever reported. We further extract the intrinsic contact resistance of low work function metal Ti on monolayer CVD MoS2 with an expectation value of 175 {\Omega}.mm, which can be significantly decreased to 10 {\Omega}.mm by appropriate gating. Finally, field-effect mobilities ({\mu}FE) of the carriers at various channel lengths are obtained. By taking the impact of contact resistance into account, an average and maximum intrinsic {\mu}FE is estimated to be 13.0 and 21.6 cm2/Vs in monolayer CVD MoS2 films, respectively.",1303.0776v1 2014-10-17,Anisotropic strain in SmSe and SmTe: implications for electronic transport,"Mixed valence rare-earth samarium compounds SmX (X=Se,Te) have been recently proposed as candidate materials for use in high-speed, low-power digital switches driven by stress induced changes of resistivity. At room temperature these materials exhibit a pressure driven insulator-to-metal transition with resistivity decreasing by up to 7 orders of magnitude over a small pressure range. Thus, the application of only a few GPa's to the piezoresistor (SmX) allows the switching device to perform complex logic. Here we study from first principles the electronic properties of these compounds under uniaxial strain and discuss the consequences on carrier transport. The changes in the band structure show that the piezoresistive response is mostly governed by the reduction of band gap with strain. Furthermore, it becomes optimal when the Fermi level is pinned near the localized valence band. The piezoresistive effect under uniaxial strain which must be taken into account in thin films and other systems with reduced dimensionality is also quantified. Under uniaxial strain we find that the piezoresistive response can be substantially larger than in the isotropic case. Analysis of complex band structure of SmSe yields a tunneling length of the order of 1 nm. The results suggest that the conduction mechanism governing the piezoresistive effect in bulk, i.e.~thermal promotion of electrons, should still be dominant in few-nanometer-thick films.",1410.4740v1 2015-08-19,Independent tuning of electronic properties and induced ferromagnetism in topological insulators with heterostructure approach,"The quantum anomalous Hall effect (QAHE) has been recently demonstrated in Cr- and V-doped three-dimensional topological insulators (TIs) at temperatures below 100 mK. In those materials, the spins of unfilled d-electrons in the transition metal dopants are exchange coupled to develop a long-range ferromagnetic order, which is essential for realizing QAHE. However, the addition of random dopants does not only introduce excess charge carriers that require readjusting the Bi/Sb ratio, but also unavoidably introduces paramagnetic spins that can adversely affect the chiral edge transport in QAHE. In this work, we show a heterostructure approach to independently tune the electronic and magnetic properties of the topological surface states in (BixSb1-x)2Te3 without resorting to random doping of transition metal elements. In heterostructures consisting of a thin (BixSb1-x)2Te3 TI film and yttrium iron garnet (YIG), a high Curie temperature (~ 550 K) magnetic insulator, we find that the TI surface in contact with YIG becomes ferromagnetic via proximity coupling which is revealed by the anomalous Hall effect (AHE). The Curie temperature of the magnetized TI surface ranges from 20 to 150 K but is uncorrelated with the Bi fraction x in (BixSb1-x)2Te3. In contrast, as x is varied, the AHE resistivity scales with the longitudinal resistivity. In this approach, we decouple the electronic properties from the induced ferromagnetism in TI. The independent optimization provides a pathway for realizing QAHE at higher temperatures, which is important for novel spintronic device applications.",1508.04719v1 2016-11-08,Superconductivity Induced by High Pressure in Weyl Semimetal TaP,"Weyl semimetal defines a material with three dimensional Dirac cones which appear in pair due to the breaking of spatial inversion or time reversal symmetry. Superconductivity is the state of quantum condensation of paired electrons. Turning a Weyl semimetal into superconducting state is very important in having some unprecedented discoveries. In this work, by doing resistive measurements on a recently recognized Weyl semimetal TaP under pressure up to about 100 GPa, we observe superconductivity at about 70 GPa. The superconductivity retains when the pressure is released. The systematic evolutions of resistivity and magnetoresistance with pressure are well interpreted by the relative shift between the chemical potential and paired Weyl points. Calculations based on the density functional theory also illustrate the structure transition at about 70GPa, the phase at higher pressure may host superconductivity. Our discovery of superconductivity in TaP by pressure will stimulate further study on superconductivity in Weyl semimetals.",1611.02548v1 2017-02-15,On Ni-Sb-Sn based skutterudites,"Novel filled skutterudites EpyNi4Sb12-xSnx (Ep = Ba and La) have been prepared by arc melting followed by annealing at 250C, 350C and 450C up to 30 days in sealed quartz vials. A maximum filling level of y = 0.93 and y = 0.65 was achieved for the Ba and La filled skutterudite, respectively. Single-phase samples with the composition Ni4Sb8.2Sn3.8, Ba0.42Ni4Sb8.2Sn3.8 and Ba0.92Ni4Sb6.7Sn5.3 were employed for measurements of the physical properties i.e. temperature dependent electrical resistivity, Seebeck coefficient and thermal conductivity. Resistivity data showed a crossover from metallic to semiconducting behaviour. The corresponding gap width was extracted from maxima in the Seebeck coefficient data as a function of temperature. Temperature dependent single crystal X-ray structure analyses (at 100 K, 200 K and 300 K) revealed the thermal expansion coefficients, Einstein and Debye temperatures for two selected samples Ba0.73Ni4Sb8.1Sn3.9 and Ba0.95Ni4Sb6.1Sn5.9. These data compare well with Debye temperatures from measurements of specific heat (4.4 K < T < 200 K). Several mechanical properties were measured and evaluated. Thermal expansion coefficients are 11.8.10-6 K-1 for Ni4Sb8.2Sn3.8 to 13.8.10-6 K-1 for Ba0.92Ni4Sb6.7Sn5.3. Room temperature Vicker's hardness values (up to a load of 24.5 mN) vary within the range of 2.6 GPa to 4.7 GPa. Severe plastic deformation (SPD) via high-pressure torsion (HPT) was used to introduce nanostructuring. Physical properties before and after HPT were compared, showing no significant effect on the material's thermoelectric behaviour.",1702.04654v1 2018-04-13,Tuning spin one channel to exotic orbital two-channel Kondo effect in ferrimagnetic composites of LaNiO3 and CoFe2O4,"We report the tuning from spin one channel (1CK) to orbital two-channel Kondo (2CK) effect by varying CoFe2O4 (CFO) content in the composites with LaNiO3 (LNO) along with the presence of ferrimagnetism. Although there is no signature of resistivity upturn in case of pure LNO, all the composites exhibit a distinct upturn in the temperature range 30-80 K. For composite with lower percentage of CFO (10 %), the electron spin plays the key role in the emergence of resistivity upturn which is affected by external magnetic field. On the other hand, when the CFO content is increased (15%), the upturn shows strong robustness against high magnetic field (14 T) and a crossover in temperature variation from lnT to T^1/2 at the Kondo temperature, indicating the appearance of orbital 2CK effect. The orbital 2CK effect is originated due to the scattering of conduction electrons from the structural two-level systems which is created at the interfaces between the two phases (LNO and CFO) of different crystal structures as well as inside the crystal planes. A negative magnetoresistance (MR) is observed at low temperature (< 30 K) for composites containing both lower (10 %) and higher percentage (15 %) of CFO. We have analyzed the negative MR using Khosla and Fisher semi-empirical model based on spin dependent scattering of conduction electrons from localized spins.",1804.04796v1 2018-06-20,Tunable disorder and localization in the rare-earth nickelates,"The rare-earth nickelates are a rich playground for transport properties, known to host non-Fermi liquid character, resistance saturation and metal-insulator transitions. We report a study of transport in LaNiO3 in the presence of tunable disorder induced by irradiation. While pristine LaNiO3 samples are metallic, highly irradiated samples show insulating behaviour at all temperatures. Using irradiation fluence as a tuning handle, we uncover an intermediate region hosting a metal-insulator transition. This transition falls within the Mott-Ioffe-Regel regime wherein the mean free path is comparable to lattice spacing. In the high temperature metallic regime, we find a transition from non-Fermi liquid to a Fermi-liquid-like character. On the insulating side of the metal-insulator transition, we find behaviour that is consistent with weak localization. This is reflected in magnetoresistance that scales with the square of the field and in resistivity. In the highly irradiated insulating samples, we find good agreement with variable range hopping, consistent with Anderson localization. We find qualitatively similar behaviour in thick PrNiO3 films as well. Our results demonstrate that ion irradiation can be used to tailor transport, serving as an excellent tool to study the physics of localization.",1806.07986v1 2019-09-04,Exploring Disorder in the Spin Gapless Semiconductor Mn$_2$CoAl,"Since the prediction of spin-gapless semiconducting behaviour in the Heusler compound Mn$_2$CoAl, evidence of spin-gapless behaviour in thin films has typically been inferred from magnetotransport measurements. The spin gapless state is however fragile, and further, band structure calculations indicate that even a small amount of atomic disorder may destroy it. To explore the impact of disorder on the properties of Mn$_2$CoAl, we have undertaken an experimental study of the structural, magnetotransport and optical properties from the far infrared to the UV, on DC magnetron sputtered Mn$_2$CoAl thin films. A very short mean free path, of the order of a lattice spacing, is extracted from the DC transport data. A room temperature resistivity of 200 $\mu$$\Omega$cm along with a small and negative temperature coefficient of resistance between 4 and 400 K was measured. We note that parameters of this magnitude are often observed in disordered metals. We find this behaviour is well described by a weak localisation model, a result that is supported by a large Drude contribution to the optical response, where a high scattering rate is derived, which is equal to the value derived from the DC conductivity and Hall effect data. We also note the strong similarities between the magnetotransport behaviour reported for Mn$_2$CoAl films in the literature, including ours. We conclude that, based on comparisons between the experimental data, and recent band structure calculations that explicitly include disorder, as-prepared Mn$_2$CoAl films are best described as a disordered metal, rather than a spin gapless semiconductor.",1909.02153v1 2019-07-10,Electronic Transport Evidence for Topological Nodal-Line Semimetals of ZrGeSe single crystals,"Although the band topology of ZrGeSe has been studied via magnetic torque technique, the electronic transport behaviors related to the relativistic Fermions in ZrGeSe are still unknown. Here, we first report systematic electronic transport properties of high-quality ZrGeSe single crystals under magnetic fields up to 14 T. Resistivity plateaus of temperature dependent resistivity curves both in the presence and absence of magnetic fields as well as large, non-saturating magnetoresistance in low-temperature region were observed. By analyzing the temperature- and angular-dependent Shubnikov-de Haas oscillations and fitting it via the Lifshitz-Kosevich (LK) formula with the Berry phase being taken into account, we proved that Dirac fermions dominate the electronic transport behaviors of ZrGeSe and the presence of non-trivial Berry phase. First principles calculations demonstrate that ZrGeSe possesses Dirac bands and normal bands near Fermi surface, resulting in the observed magnetotransport phenomena. These results demonstrate that ZrGeSe is a topological nodal-line semimetal, which provides a fundamentally important platform to study the quantum physics of topological semimetals.",1907.04762v1 2019-12-06,Correlated Insulating States and Transport Signature of Superconductivity in Twisted Trilayer Graphene Moiré of Moiré Superlattices,"Layers of two-dimensional materials stacked with a small twist-angle give rise to beating periodic patterns on a scale much larger than the original lattice, referred to as a moir\'e superlattice. When the stacking involves more than two layers with independent twist angles between adjacent layers, it generates moir\'e of moir\'e superlattices, with multiple length scales that control the system's behavior. Here we demonstrate these effects of a high-order moir\'e superlattice in twisted trilayer graphene with two consecutive small twist angles. We report correlated insulating states near the half filling of the moir\'e of moir\'e superlattice at an extremely low carrier density (~1010 cm-2), near which we also report a zero-resistance transport behavior typically expected in a 2D superconductor. Moreover, the temperature dependence of the measured resistances at full-occupancy (v = -4 and v = 4) states are semi-metallic, distinct from the insulating behavior of twisted bilayer systems, providing the first demonstration of emergent correlated transport behaviors from continuous, non-isolated higher-order moir\'e flat bands. Our findings shed new insights into the microscopic mechanisms of moir\'e correlated states and provide the impetus for future studies on this material platform, such as the demonstration of phase coherence and Meissner-like effect.",1912.03375v2 2020-01-14,Heavy non-degenerate electrons in doped strontium titanate,"Room-temperature metallicity of lightly doped SrTiO$_3$ is puzzling, because the combination of mobility and the effective mass would imply a mean-free-path (mfp) below the Mott Ioffe Regel (MIR) limit and a scattering time shorter than the Planckian time ($\tau_P=\hbar/k_BT$). We present a study of electric resistivity, Seebeck coefficient and inelastic neutron scattering extended to very high temperatures, which deepens the puzzle. Metallic resistivity persists up to 900 K and is accompanied by a large Seebeck coefficient whose magnitude (as well as its temperature and doping dependence) indicates that carriers are becoming heavier with rising temperature. Combining this with neutron scattering data, we find that between 500 K and 900 K, the Bohr radius and the electron wave-length become comparable to each other and twice the lattice parameter. According to our results, between 100 K and 500 K, metallicity is partially driven by temperature-induced amplification of the carrier mass. We contrast this mass amplification of non-degenerate electrons with the better-known case of heavy degenerate electrons. Above 500 K, the mean-free-path continues to shrink with warming in spite of becoming shorter than both the interatomic distance and the thermal wavelength of the electrons. The latter saturates to twice the lattice parameter. Available theories of polaronic quasi-particles do not provide satisfactory explanation for our observations.",2001.04668v4 2021-06-21,Three-dimensional quasi-quantized Hall insulator phase in SrSi2,"In insulators, the longitudinal resistivity becomes infinitely large at zero temperature. For classic insulators, the Hall conductivity becomes zero at the same time. However, there are special systems, such as two-dimensional quantum Hall isolators, in which a more complex scenario is observed at high magnetic fields. Here, we report experimental evidence for a quasi-quantized Hall insulator in the quantum limit of the three-dimensional semimetal SrSi2. Our measurements reveal a magnetic field-range, in which the longitudinal resistivity diverges with decreasing temperature, while the Hall conductivity approaches a quasi-quantized value that is given only by the conductance quantum and the Fermi wave vector in the field-direction. The quasi-quantized Hall insulator appears in a magnetic-field induced insulating ground state of three-dimensional materials and is deeply rooted in quantum Hall physics.",2106.11329v1 2021-07-05,Quantum anomalous Hall effect from intertwined moiré bands,"Electron correlation and topology are two central threads of modern condensed matter physics. Semiconductor moir\'e materials provide a highly tunable platform for studies of electron correlation. Correlation-driven phenomena, including the Mott insulator, generalized Wigner crystals, stripe phases and continuous Mott transition, have been demonstrated. However, nontrivial band topology has remained elusive. Here we report the observation of a quantum anomalous Hall (QAH) effect in AB-stacked MoTe2/WSe2 moir\'e heterobilayers. Unlike in the AA-stacked structures, an out-of-plane electric field controls not only the bandwidth but also the band topology by intertwining moir\'e bands centered at different high-symmetry stacking sites. At half band filling, corresponding to one particle per moir\'e unit cell, we observe quantized Hall resistance, h/e2 (with h and e denoting the Planck's constant and electron charge, respectively), and vanishing longitudinal resistance at zero magnetic field. The electric-field-induced topological phase transition from a Mott insulator to a QAH insulator precedes an insulator-to-metal transition; contrary to most known topological phase transitions, it is not accompanied by a bulk charge gap closure. Our study paves the path for discovery of a wealth of emergent phenomena arising from the combined influence of strong correlation and topology in semiconductor moir\'e materials.",2107.01796v1 2021-10-01,Gate-tunable Intrinsic Anomalous Hall Effect in Epitaxial MnBi2Te4 Films,"Anomalous Hall effect (AHE) is an important transport signature revealing topological properties of magnetic materials and their spin textures. Recently, antiferromagnetic MnBi2Te4 has been demonstrated to be an intrinsic magnetic topological insulator that exhibits quantum AHE in exfoliated nanoflakes. However, its complicated AHE behaviors may offer an opportunity for the unexplored correlation between magnetism and band structure. Here, we show the Berry curvature dominated intrinsic AHE in wafer-scale MnBi2Te4 thin films. By utilizing a high-dielectric SrTiO3 as the back-gate, we unveil an ambipolar conduction and electron-hole carrier (n-p) transition in ~7 septuple layer MnBi2Te4. A quadratic relation between the saturated AHE resistance and longitudinal resistance suggests its intrinsic AHE mechanism. For ~3 septuple layer MnBi2Te4, however, the AHE reverses its sign from pristine negative to positive under the electric-gating. The first-principles calculations demonstrate that such behavior is due to the competing Berry curvature between polarized spin-minority-dominated surface states and spin-majority-dominated inner-bands. Our results shed light on the physical mechanism of the gate-tunable intrinsic AHE in MnBi2Te4 thin films and provide a feasible approach to engineering its AHE.",2110.00540v1 2021-12-23,Impact of the superconductors properties on the measurement sensitivity of resonant-based axion detectors,"Axions, hypothetical particles theorized to solve the strong CP-problem, are presently being considered as strong candidates as cold dark matter constituents. The signal power of resonant-based axion detectors, known as haloscopes, is directly proportional to their quality factor $Q$. In this paper, the impact of the use of superconductors in the performances of the haloscopes is studied by evaluating the obtainable $Q$. In particular, the surface resistance $R_s$ of NbTi, Nb$_3$Sn, YBa$_2$Cu$_3$O$_{7-\delta}$ and FeSe$_{0.5}$Te$_{0.5}$ is computed in the frequency, magnetic field and temperature ranges of interest, starting from the measured vortex motion complex resistivity and screening lengths of these materials. From $R_s$ the quality factor $Q$ of a cylindrical haloscope with copper conical bases and superconductive lateral wall, operating with the TM$_{010}$ mode, is evaluated and used to perform a comparison of the performances of the different materials. Both YBa$_2$Cu$_3$O$_{7-\delta}$ and FeSe$_{0.5}$Te$_{0.5}$ are shown to improve the measurement sensitivity by almost an order of magnitude with respect to a whole Cu cavity, while NbTi is shown to be suitable only at lower frequencies (<10 GHz). Nb$_3$Sn can give an intermediate improvement in the whole spectrum of interest.",2112.12775v1 2022-01-28,Substitutional Doped GeSe: Tunable Oxidative States with Strain Engineering,"Layered chalcogenide materials have a wealth of nanoelectronics applications like resistive switching and energy-harvesting such as photocatalyst owing to rich electronic, orbital, and lattice excitations. In this work, we explore monochalcogenide germanium selenide GeSe with respect to substitutional doping with 13 metallic cations by using first-principles calculations. Typical dopants including s-shell (alkali elements Li and Na), p-shell (Al, Pb and Bi), 3d (Fe, Cu, Co and Ni), 4d (Pd and Ag) and 5d (Au and Pt) elements are systematically examined. Amongst all the cationic dopants, Al with the highest oxidation states, implying a high mobility driven by electric field, and Al-doped GeSe may be a promising candidate for novel resistive switching devices. We show that there exist many localized induced states in the band gap of GeSe upon doping Fe, Co, or Ni, while for Cu, Ag, and Au cases there is no such states in the gap. The Ag and Cu are + 0.27 and + 0.35 charged respectively and the positive charges are beneficial for field-driven motion in GeSe. In contrast, Au is slightly negatively charged renders Au-doped GeSe a promising photocatalyst and enhanced surface plasmon. Moreover, we explore the coexistence of dopant and strain in GeSe and find dynamical adjustments of localized states in GeSe with levels successive shifting upward/downward with strain. This induces dynamic oxidative states of the dopants under strain which should be quite popular in composites where motion of metal adatoms causes significant deformation.",2201.11890v1 2022-05-24,Quantum hybridization negative differential resistance from non-toxic halide perovskite nanowire heterojunctions and its strain control,"While low-dimensional organometal halide perovskites are expected to open up new opportunities for a diverse range of device applications, like in their bulk counterparts, the toxicity of Pb-based halide perovskite materials is a significant concern that hinders their practical use. We recently predicted that lead triiodide (PbI$_3$) columns de-rived from trimethylsulfonium (TMS) lead triiodide (CH$_3$)$_3$SPbI$_3$ (TMSPbI$_3$) by stripping off TMS ligands should be semimetallic, and additionally ultrahigh negative differential resistance (NDR) can arise from the heterojunction composed of a TMSPbI$_3$ channel sandwiched by PbI$_3$ electrodes. Herein, we computationally explore whether similar material and device characteristics can be obtained from other one-dimensional halide perovskites based on non-Pb metal elements, and in doing so deepen the understanding of their mechanistic origins. First, scanning through several candidate metal halide inorganic frameworks as well as their parental form halide perovskites, we find that the germanium triiodide (GeI$_3$) column also assumes a semimetallic character by avoiding the Peierls distortion. Next, adopting the bundled nanowire GeI$_3$-TMSGeI$_3$-GeI$_3$ junction configuration, we obtain a drastically high peak current density and ultrahigh NDR at room temperature. Furthermore, the robustness and controllability of NDR signals under strain are revealed, establishing its potential for flexible electronics applications. It will be emphasized that, despite the performance metrics notably enhanced over those from the PbI$_3$-TMSPbI$_3$-PbI$_3$ case, these device characteristics still arise from the identical quantum hybridization NDR mechanism.",2205.11689v1 2022-06-06,"Anisotropic magnetic property of single crystals $R$V$_6$Sn$_6$ ($R$ = Y, Gd - Tm, Lu)","$R$V${_6}$Sn${_6}$ ($R$ = Y, Gd - Tm, Lu) single crystals are synthesized by Sn-flux method and their physical properties are characterized by magnetization, resistivity, and specific heat measurements. Powder X-ray diffraction patterns of all samples can be well indexed with the hexagonal HfFe$_6$Ge$_6$-type structure, where rare-earth atoms form hexagonal layers and vanadium atoms form Kagome layers. At high temperatures, magnetic susceptibility measurements of moment bearing rare-earths ($R$ = Gd - Tm) follow Curie-Weiss behavior. Effective moments estimated from the polycrystalline average of magnetic susceptibility curves are consistent with the values for free $R^{3+}$ ion. Strong magnetic anisotropy due to crystalline electric field effects is observed for moment bearing rare-earths, except GdV$_6$Sn$_6$. The easy magnetization direction is determined to be $c$-axis for $R$ = Tb - Ho and $ab$-plane for $R$ = Er, and Tm. The vanadium ions in $R$V${_6}$Sn${_6}$ possess no magnetic moment. The compounds for $R$ = Y and Lu exhibit typical characteristics of paramagnetic metals. At low temperatures, the magnetic ordering is confirmed from magnetization, specific heat, and resistivity: the highest $T_{N} = 4.9$~K for GdV$_6$Sn$_6$ and the lowest $T_{N} = 2.3$~K for HoV$_6$Sn$_6$. No magnetic ordering is observed down to 1.8~K for $R$ = Er and Tm. A slight deviation of the magnetic ordering temperature from the de Gennes scaling suggests the dominant Ruderman-Kittel-Kasuya-Yosida (RKKY) exchange interaction between rare-earth moments in metallic $R$V${_6}$Sn${_6}$ compounds.",2206.02924v1 2022-09-21,Optical properties and carrier localization in the layered phosphide EuCd$_\mathbf{2}$P$_\mathbf{2}$,"The temperature dependence of the complex optical properties of the layered phosphide material EuCd$_2$P$_2$ have been measured over a wide frequency range above and below $T_{\rm N} \simeq 11.5$ K for light polarized in the $a-b$ planes. At room temperature, the optical conductivity is well described by a weak free-carrier component with a Drude plasma frequency of $\simeq 1100$ cm$^{-1}$ and a scattering rate of $1/\tau_D\simeq 700$ cm$^{-1}$, with the onset of interband absorptions above $\simeq 2000$ cm$^{-1}$. Two infrared-active $E_u$ modes are observed at $\simeq\,$89 and 239 cm$^{-1}$. As the temperature is reduced the scattering rate decreases and the low-frequency conductivity increases slightly; however, below $\simeq 50$ K the conductivity decreases until at the resistivity maximum at $\simeq 18$ K (just below $2T_{\rm N}$) the spectral weight associated with free carriers is transferred to a localized excitation at $\simeq 500$ cm$^{-1}$. Below $T_{\rm N}$, metallic behavior is recovered. Interestingly, the $E_u$ modes are largely unaffected by these changes, with only the position of the high-frequency mode showing any signs of anomalous behavior. While several scenarios are considered, the prevailing view is that the resistivity maximum and subsequent carrier localization is due to the formation of ferromagnetic domains below $\simeq 2T_{\rm N}$ that result in spin-polarized clusters due to spin-carrier coupling [1].",2209.10606v2 2022-10-14,Anti-site disorder and Berry curvature driven anomalous Hall effect in spin gapless semiconducting Mn2CoAl Heusler compound,"Spin gapless semiconductors exhibit a finite band gap for one spin channel and closed gap for other spin channel, emerged as a new state of magnetic materials with a great potential for spintronic applications. The first experimental evidence for the spin gapless semiconducting behavior was observed in an inverse Heusler compound Mn2CoAl. Here, we report a detailed investigation of the crystal structure and anomalous Hall effect in the Mn2CoAl using experimental and theoretical studies. The analysis of the high-resolution synchrotron x-ray diffraction data shows anti-site disorder between Mn and Al atoms within the inverse Heusler structure. The temperature-dependent resistivity shows semiconducting behavior and follows Mooijs criteria for disordered metal. Scaling behavior of the anomalous Hall resistivity suggests that the anomalous Hall effect in the Mn2CoAl is primarily governed by intrinsic mechanism due to the Berry curvature in momentum space. The experimental intrinsic anomalous Hall conductivity (AHC) is found to be 35 S/cm, which is considerably larger than the theoretically predicted value for ordered Mn2CoAl. Our first-principle calculations conclude that the anti-site disorder between Mn and Al atoms enhances the Berry curvature and hence the value of intrinsic AHC, which is in a very well agreement with the experiment.",2210.07668v1 2022-12-02,FeRhCrSi: A new spin semimetal with room temperature spin-valve behavior,"Spin semimetals are a recently discovered new class of spintronic materials, which exhibit a band gap in one spin channel while a semimetallic feature in the other and thus allows for tunable spin transport. Here, we present experimental verification of spin semimetallic behavior in FeRhCrSi, a quaternary Heusler alloy with saturation moment 2 $\mu_B$ and Curie temperature $>$ 400 K. It crystallises in the L2$_1$ structure with 50$\%$ antisite disorder between Fe and Rh. Below 300 K, it shows a weakly temperature dependent electrical resistivity with negative temperature coefficient, indicating the normal semimetal or spin semimetal behavior. Anomalous magnetoresistance data reveals dominant contribution from asymmetric part, a clear signature of spin-valve nature, which is retained even at room temperature. \textcolor{black}{The asymmetric part of magneto-resistance shows an unusual increase with increasing temperature.} Hall measurements confirm the anomalous nature of conductivity originating from the intrinsic Berry curvature, with holes being the majority carriers. Ab-initio simulation confirms a unique long-range ferrimagnetic ordering to be the ground state, explaining the origin behind the unexpected low saturation moment. The ferrimagnetic disordered structure confirms the spin semimetallic feature of FeRhCrSi, as observed experimentally.",2212.00924v2 2023-01-11,Domain Wall-Magnetic Tunnel Junction Analog Content Addressable Memory Using Current and Projected Data,"With the rise in in-memory computing architectures to reduce the compute-memory bottleneck, a new bottleneck is present between analog and digital conversion. Analog content-addressable memories (ACAM) are being recently studied for in-memory computing to efficiently convert between analog and digital signals. Magnetic memory elements such as magnetic tunnel junctions (MTJs) could be useful for ACAM due to their low read/write energy and high endurance, but MTJs are usually restricted to digital values. The spin orbit torque-driven domain wall-magnetic tunnel junction (DW-MTJ) has been recently shown to have multi-bit function. Here, an ACAM circuit is studied that uses two domain wall-magnetic tunnel junctions (DW-MTJs) as the analog storage elements. Prototype DW-MTJ data is input into the magnetic ACAM (MACAM) circuit simulation, showing ternary CAM function. Device-circuit co-design is carried out, showing that 8-10 weight bits are achievable, and that designing asymmetrical spacing of the available DW positions in the device leads to evenly spaced ACAM search bounds. Analyzing available spin orbit torque materials shows platinum provides the largest MACAM search bound while still allowing spin orbit torque domain wall motion, and that the circuit is optimized with minimized MTJ resistance, minimized spin orbit torque material resistance, and maximized tunnel magnetoresistance. These results show the feasibility of using DW-MTJs for MACAM and provide design parameters.",2301.04598v1 2023-04-26,Microbial Corrosion Prevention by Citrobacter sp. Biofilms,"Microbiologically influenced corrosion (MIC) compromises the integrity of many technologically relevant metals. Protective coatings based on synthetic materials pose potential environmental impacts. Here, we report a MIC resistant coating based on a biofilm matrix of Citrobacter sp. strain MIC21 on underlying copper (Cu) surfaces. Three identical corrosion cells varying in the type of working electrode (annealed Cu, 29.5% coldworked, and 56.2% coldworked Cu) were used. Graphite plate and Ag/AgCl served as counter and reference electrodes, respectively. The working electrolyte was based on lactate-C media along with an inocula consisting of Oleidesulfovibrio alaskensis strain G20 and Citrobacter sp. strain MIC21. Passivating effect of the co-cultured biofilm matrix was observed in the form of an ennoblement effect. Tests based on sequencing, microscopy, and spectroscopy revealed the formation of a compact biofilm matrix dominated by strain MIC21 cells, exopolymers, and insoluble precipitates. This matrix displayed elastic modulus (a measure of rigidity) as high as 0.8 Gpa and increased corrosion resistance by ~10-fold. Interestingly, strain MIC21 has the capacity to inhibit the undesirable growth of aggressive strain G20. Additional corrosion tests also substantiated the passivation effects of strain MIC21. We provide mechanistic insight into the underlying reasons responsible for corrosion prevention behavior of the biofilm matrix.",2304.13862v1 2023-06-01,Bulk conducting states of intrinsically doped Bi$_2$Se$_3$,"With a large band gap and a single Dirac cone responsible for the topological surface states, Bi2Se3 is widely regarded as a prototypical 3D topological insulator. Further applications of the bulk material has, however, been hindered by inherent structural defects that donate electrons and make the bulk conductive. Consequently, controlling these defects is of great interest for future technological applications, and while past literature has focused on adding external doping elements to the mixture, a complete study on undoped Bi2Se3 was still lacking. In this work, we use the self-flux method to obtain high-quality Bi2Se3 single-crystals in the entire concentration range available on the phase-diagram for the technique. By combining basic structural characterization with measurements of the resistivity, Hall effect and Shubnikov-de Haas (SdH) quantum oscillations, the effects of these impurities on the bulk transport are investigated in samples with electron densities ranging from 10^17 cm^-3 to 10^19 cm^-3, from Se-rich to Bi-rich mixtures, respectively, evidencing the transition into a degenerate semiconductor regime. We find that electron-donor impurities, likely Se vacancies, unavoidably shift the Fermi level up to 200 meV inside the conduction band. Other impurities, like interstitial Bi and Se, are shown to play a significant role as scattering centres, specially at low temperatures and in the decoherence of the SdH oscillations. Previous open questions on Bi2Se3, such as the upturn in resistivity below 30 K, the different scattering times in transport and quantum oscillations, and the presence of additional low mobility bands, are addressed. The results outlined here provide a concise picture on the bulk conducting states in flux-grown Bi2Se3 single crystals, enabling better control of the structural defects and electronic properties.",2306.00827v1 2023-07-06,"Tunable magnetism and electron correlation in Titanium-based Kagome metals RETi3Bi4 (RE = Yb, Pr, and Nd) by rare-earth engineering","Rare-earth engineering is an effective way to introduce and tune the magnetism in topological Kagome magnets, which has been acting as a fertile platform to investigate the quantum interactions between geometry, topology, spin, and correlation. Here we report the structure and properties of three newly discovered Titanium-based Kagome metals RETi3Bi4 (RE = Yb, Pr, and Nd) with various magnetic states. They crystalize in the orthogonal space group Fmmm (No.69), where slightly distorted Ti Kagome lattice, RE triangular lattice, Bi honeycomb and triangular lattices stack along the a axis. By changing the rare earth atoms on RE zag-zig chains, the magnetism can be tuned from nonmagnetic YbTi3Bi4 to short-range ordered PrTi3Bi4 (Tanomaly ~ 8.2 K), and finally to ferromagnetic NdTi3Bi4 (Tc ~ 8.5 K). The measurements of resistivity and specific heat capacity demonstrate an evolution of electron correlation and density of states near the Fermi level with different rare earth atoms. In-situ resistance measurements of NdTi3Bi4 under high pressure further reveal a potential relationship between the electron correlation and ferromagnetic ordering temperature. These results highlight RETi3Bi4 as another family of topological Kagome magnets to explore nontrivial band topology and exotic phases in Kagome materials.",2307.02942v1 2023-09-23,Three-dimensional graphene on a nano-porous 4H-SiC backbone: a novel material for food sensing applications,"Sensors which are sensitive to volatile organic compounds and thus able to monitor the conservation state of food, are precious because they work non-destructively and allow to avoid direct contact with the food, ensuring hygienic conditions. In particular, the monitoring of rancidity would solve a widespread issue in food storage. The sensor discussed here is produced utilizing a novel three-dimensional arrangement of graphene, which is grown on a crystalline silicon carbide (SiC) wafer previously porousified by chemical etching. This approach allows a very high surface-to.volume ratio. Furthermore, the structure of the sensor surface features a large amount of edges, dangling bounds, and active sites, which make the sensor, on a chemically robust skeleton, chemically active, particularly to hydrogenated molecules. The interaction of the sensor with such compounds is read out by measuring the sensor resistance in a four wire configuration. The sensor performance has been assessed on three hazelnut samples: sound hazelnuts, spoiled hazelnuts, and stink bug hazelnuts. A resistance variation of about DeltaR = 0.13 (0.02) Ohm between sound and damaged hazelnuts has been detected. Our measurements confirm the ability of the sensor to discriminate between sound and damaged hazelnuts. The sensor signal is stable for days, providing the possibility to use this sensor for the monitoring of the storage state of fats and foods in general.",2309.13431v1 2023-09-26,On Hyperelastic Crease,"We present analyses of crease-formation and stability criteria for incompressible hyperelastic solids. A generic singular perturbation over a laterally compressed half-space creates a far-field eigenmode of three energy-release angular sectors separated by two energy-elevating sectors of incremental deformation. The far-field eigenmode braces the energy-release field of the surface flaw against the transition to a self-similar crease field, and the braced-incremental-deformation (bid) field has a unique shape factor that determines the creasing stability. The shape factor, which is identified by two conservation integrals that represent a subsurface dislocation in the tangential manifold, is a monotonically increasing function of compressive strain. For Neo-Hookean material, when the shape factor is below unity, the bid field is configurationally stable. When the compressive strain is 0.356, the shape factor becomes unity, and the bid field undergoes a higher-order transition to a crease field. At the crease-limit point, we have two asymptotic solutions of the crease-tip folding field and the leading-order far field with two scaling parameters, the ratio of which is determined by matched asymptotes. Our analyses show that the surface is stable against singular perturbation up to the crease limit point and becomes unstable beyond the limit. However, the flat state is metastable against a regular perturbation between the crease limit point and wrinkle critical point, which is a first-order instability point. We introduced a novel finite element method for simulating the bid field with a finite domain size. For Gent model, the strain-stiffening alters the shape factor dependence on the compressive strain, raising crease resistance. The new findings in crease mechanisms will help study ruga mechanics of self-organization and design soft-material structures for high crease resistance.",2309.14626v1 2024-02-15,Quantum Linear Magnetoresistance and Fermi Liquid Behavior in Kagome Metal Ni3In2S2,"Kagome metals gain attention as they manifest a spectrum of quantum phenomena, including superconductivity, charge order, frustrated magnetism, and intertwined correlated states of condensed matter. With regard to electronic band structure, several of the them exhibit non-trivial topological characteristics. Here, we present a thorough investigation on the growth and the physical properties of single crystals of Ni3In2S2 which is established to be a Dirac nodal line Kagome metal. Extensive characterization is attained through temperature and field-dependent resistivity, angle-dependent magnetoresistance and specific heat measurements. In most metals, the Fermi liquid behaviour is mostly restricted to a narrow range of temperature. In Ni3In2S2, this characteristic feature has been observed for an extensive temperature range of 82 K. This is attributed to the strong electron-electron correlation in the material. Specific heat measurements reveal a high Kadowaki-Woods ratio which is in good agreement with strongly correlated systems. Almost linear positive magnetoresistance follows the conventional Kohler scaling which depicts the applicability of semi-classical theories. The angle-dependent magneto-resistance been explained using the Voigt-Thomson formula. Furthermore, de-Haas van Alphen oscillations are observed in magnetization vs. magnetic field measurement which shed light on the topological features in the Shandite Ni3In2S2.",2402.10096v1 2022-11-28,On the energy conversion efficiency of the bulk photovoltaic effect,"The bulk photovoltaic effect (BPVE) leads to directed photo-currents and photo-voltages in bulk materials. Unlike photo-voltages in p-n junction solar cells that are limited by carrier recombination to values below the bandgap energy of the absorbing material, the BPVE photo-voltages have been shown to greatly exceed the bandgap energy. Therefore the BPVE is not subject to the Shockley-Queisser limit for sunlight to electricity conversion in single junction solar cells and experimental claims of efficiencies beyond this limit have been made. Here, we show that BPVE energy conversion efficiencies are, in practice, orders of magnitude below the Shockley-Queisser limit of single junction solar cells and are subject to different, more stringent limits. The name BPVE stands for two different fundamental effects, the shift current and the injection current. In both of these, the voltage bias necessary to produce electrical energy, accelerates both, intrinsic and photo-generated, carriers. We discuss how energy conservation alone fundamentally limits the BPVE to a bandgap-dependent value that exceeds the Shockley Queisser limit only for very small bandgaps. Yet, small bandgap materials have a large number of intrinsic carriers, leading to high conductivity which suppresses the photo-voltage. We discuss further how slightly more stringent fundamental limits for injection (ballistic) currents may be derived from the trade-off between high resistivity, needed for a high voltage, and long ballistic transport length, needed for a high current. We also explain how erroneous experimental and theoretical claims of high efficiency have arisen. Finally, we calculate the energy conversion efficiency for an example 2D material that has been suggested as candidate material for high efficiency BPVE based solar cells and show that the efficiency is very similar to the efficiency of known 3D materials.",2211.15124v2 2016-07-06,Thermal Resistances of Thin-Films of Small Molecule Organic Semiconductors,"We have measured the thermal resistances of thin films of the small molecule organic semiconductors bis(triisopropylsilylethynyl) pentacene (TIPS-pn), bis(triethylsilylethynyl) anthradithiophene (TES-ADT) and difluoro bis(triethylsilylethynyl) anthradithiophene (diF-TES-ADT). For each material, several films of different thicknesses have been measured to separate the effects of intrinsic thermal conductivity from interface thermal resistance. For non-crystalline films of all three materials, with thicknesses ranging from < 100 nm to > 4 microns, the thermal conductivities are similar to that of polymers and over an order of magnitude smaller than that of the crystals, reflecting the large reduction in phonon mean-free path in the films. Thin (< 205 nm) crystalline films of TES-ADT, prepared by vapor-annealing spin-cast films, have also been measured, but for these the thermal resistances are dominated by interface scattering.",1607.01712v2 2012-06-11,Thermal Stability of Thermoelectric Materials via In Situ Resistivity Measurements,"An experimental setup for determining the electrical resistivity of several types of thermoelectric materials over the temperature range 20 < T < 550 C is described in detail. One resistivity measurement during temperature cycling is also explained for Cu0.01Bi2Te2.7Se0.3 while a second measurement is made on Yb0.35Co4Sb12 as a function of time at 400 C. Both measurements confirm that the materials are thermally stable for the temperature range and time period measured. Measurements made during temperature cycling show an irreversible decrease in the electrical resistivity of Cu0.01Bi2Te2.7Se0.3 when the measuring temperature exceeds the pressing temperature. Several other possible uses of such a system include but are not limited to studying the effects of annealing and/or oxidation as a function of both temperature and time.",1206.2094v1 2022-07-27,Terahertz microresonators for material characterisation,"Terahertz (THz) technology is rapidly evolving, and the advancement of data and information processing devices is essential. Silicon THz microresonators provide perfect platforms to develop compact and integrated devices that could transform THz technology. Here we present a systematic study on the key figure of merit of silicon THz disc microresonators - the quality factor (Q-factor) - in dependence on the substrate's resistivity. Our results show that the Q-factor depends linearly on the resistivity and a variation in resistivity from 10k$\Omega$cm to 15k$\Omega$cm changes the Q-factor from 50k to 76k at 0.6THz. Moreover, we experimentally determine that the silicon material absorption is inversely proportional to the substrate's resistivity. In general, the presented methodology is ideally suited to precisely measure the material absorption of low-loss materials in the THz domain, which is challenging using conventional THz spectroscopy.",2207.13818v1 2023-03-24,Charge-density-wave resistive switching and voltage oscillations in ternary chalcogenide BaTiS3,"Phase change materials, which show different electrical characteristics across the phase transitions, have attracted considerable research attention for their potential electronic device applications. Materials with metal-to-insulator or charge density wave (CDW) transitions such as VO2 and 1T-TaS2 have demonstrated voltage oscillations due to their robust bi-state resistive switching behavior with some basic neuronal characteristics. BaTiS3 is a small bandgap ternary chalcogenide that has recently reported the emergence CDW order below 245 K. Here, we report on the discovery of DC voltage / current-induced reversible threshold switching in BaTiS3 devices between a CDW phase and a room temperature semiconducting phase. The resistive switching behavior is consistent with a Joule heating scheme and sustained voltage oscillations with a frequency of up to 1 kHz has been demonstrated by leveraging the CDW phase transition and the associated negative differential resistance. Strategies of reducing channel sizes and improving thermal management may further improve the device performance. Our findings establish BaTiS3 as a promising CDW material for future energy-efficient electronics, especially for neuromorphic computing.",2303.14169v1 2016-02-24,Design and optimization of resistive anode for a two-dimensional imaging triple-GEM detector,"The optimization of resistive anode for two dimensional imaging detectors which consists of a series of high resistive square pads surrounding by low resistive strips has been studied by both numerical simulations and experimental tests. It has been found that to obtain good detector performance, the resistance ratio of the pad to the strip should be larger than 5, the nonuniformity of the pad surface resistivity had better be less than $20\%$, a smaller pad width leads to a smaller spatial resolution and when the pad width is $6mm$, the spatial resolution ($\sigma$) can reach about $105{\mu}m$. Based on the study results, a 2-D GEM detector prototype with the optimized resistive anode is constructed and a good imaging performance is achieved.",1602.07438v1 2017-09-19,Considering non-uniform current distributions in magnetoresistive sensor designs and their implications for the resistance transfer function,"Non-uniform current distributions of spin valves with disk shaped free layers are investigated. In the context of spin valves, the vortex state, which is the ground-state in many disk shaped magnetic bodies, allows for distinct parallel channels of high and low resistivity. The readout current is thus able to evade high resistivity regions in favor of low resistivity regions, giving rise to 'conductive inhomogeneities'. Therefore, the total resistance of the spin valve does not always correspond exactly to the total average magnetization of the free layer. In addition, the resistance transfer function can be significantly influenced by the spatial placement of the electrodes, giving rise to 'geometric inhomogeneities'. The resulting deviations from resistance to magnetization transfer function are investigated for different spin valve geometries and compared to measurements of comparable devices.",1709.06394v1 2023-09-19,Effects of plasma resistivity in three-dimensional full-F gyro-fluid turbulence simulations,"A full-F, isothermal, electromagnetic, gyro-fluid model is used to simulate plasma turbulence in a COMPASS-sized, diverted tokamak. A parameter scan covering three orders of magnitude of plasma resistivity and two values for the ion to electron temperature ratio with otherwise fixed parameters is setup and analysed. Simulations are performed with a new version of the FELTOR code, which is fully parallelized on GPUs. Each simulation covers a couple of milliseconds. Two transport regimes for high and low plasma resistivities are revealed. Beyond a critical resistivity the mass and energy confinement reduces with increasing resistivity. Further, for high plasma resistivity the direction of parallel acceleration is swapped compared to low resistivity. The integration of exact conservation laws over the closed field line region allows for an identification of numerical errors within the simulations. The electron force balance and energy conservation show relative errors on the order of $10^{-3}$ while the particle conservation and ion momentum balance show errors on the order of $10^{-2}$. Relative fluctuations amplitudes increase from below $1\%$ in the core to $15\%$ in the edge and up to $40\%$ in the scrape-off layer. Finally, three-dimensional visualisations using ray tracing techniques are displayed and discussed. The field-alignment of turbulent fluctuations in density and parallel current becomes evident.",2309.10414v1 2016-11-09,"TiO$_2$-based Memristors and ReRAM: Materials, Mechanisms and Models (a Review)","The memristor is the fundamental non-linear circuit element, with uses in computing and computer memory. ReRAM (Resistive Random Access Memory) is a resistive switching memory proposed as a non-volatile memory. In this review we shall summarise the state of the art for these closely-related fields, concentrating on titanium dioxide, the well-utilised and archetypal material for both. We shall cover material properties, switching mechanisms and models to demonstrate what ReRAM and memristor scientists can learn from each other and examine the outlook for these technologies.",1611.04456v1 2018-10-30,An alternative to the topological interpretation of the transverse resistivity anomalies in SrRuO3,"We clarify the physical origin of anomalies in transverse resistivity often observed in exotic materials, such as SrRuO3, in which the Berry curvature is manifested in the transport properties. The previously attributed mechanism for the anomalies, the topological Hall effect (THE), is refuted by our thorough investigations as well as formulation of a model considering inhomogeneous magnetoelectric properties in the material. Our analyses fully explain every feature of the anomalies without resorting to the THE. The present results establish a fundamental understanding, which was previously overlooked, of magneto-transport properties in such exotic materials.",1810.12529v1 2004-11-26,The Acceleration Mechanism of Resistive MHD Jets Launched from Accretion Disks,"We analyzed the results of non-linear resistive magnetohydrodynamical (MHD) simulations of jet formation to study the acceleration mechanism of axisymmetric, resistive MHD jets. The initial state is a constant angular momentum, polytropic torus threaded by weak uniform vertical magnetic fields. The time evolution of the torus is simulated by applying the CIP-MOCCT scheme extended for resistive MHD equations. We carried out simulations up to 50 rotation period at the innermost radius of the disk created by accretion from the torus. The acceleration forces and the characteristics of resistive jets were studied by computing forces acting on Lagrangian test particles. Since the angle between the rotation axis of the disk and magnetic field lines is smaller in resistive models than in ideal MHD models, magnetocentrifugal acceleration is smaller. The effective potential along a magnetic field line has maximum around $z \sim 0.5r_0$ in resistive models, where $r_0$ is the radius where the density of the initial torus is maximum. Jets are launched after the disk material is lifted to this height by pressure gradient force. Even in this case, the main acceleration force around the slow magnetosonic point is the magnetocentrifugal force. The power of the resistive MHD jet is comparable to the mechanical energy liberated in the disk by mass accretion. Joule heating is not essential for the formation of jets.",0411712v1 2016-10-30,Temperature and Humidity Dependence of Resistance in Nano-Diamond Powder,"The electrical resistance of detonation nano-diamond powders was measured from liquid nitrogen temperature to room temperature and in relative humidity environments from around 10% to 100%. After sample exposures of several hours at 100% relative humidity at room temperature (around 295 K), when the temperature was reduced, the resistance increased to the upper measurement limit of our apparatus (120 M{\Omega}) at around 240 K. Upon warming, the resistance dropped back to the room temperature value, with some hysteresis. For sample exposures after several hours at 100% relative humidity at room temperature, as the relative humidity was reduced, the sample resistance increased to the upper range limit of the apparatus. As the relative humidity was then increased (all at room temperature), the resistance dropped. For samples exposed to low (~10%) relative humidity for several hours at room temperature, as the humidity was increased (at room temperature), the resistance decreased, and then increased when the humidity was reduced. The temperature behavior was markedly differ from that of powdered graphite and multi-walled carbon nano tubes.",1611.02242v2 2018-07-04,Gate controlled large resistance switching driven by charge density wave in 1T-TaS2/2H-MoS2 heterojunction,"1T-TaS2 is a layered material that exhibits charge density wave (CDW) induced distinct electrical resistivity phases and has attracted a lot of attention for interesting device applications. However, such resistivity switching effects are often weak, and cannot be modulated by an external gate voltage - limiting their widespread usage. Using a back-gated 1T-TaS2/2H-MoS2 heterojunction, here we show that the usual resistivity switching in TaS2 due to different phase transitions is accompanied with a surprisingly strong modulation in the Schottky barrier height (SBH) at the TaS2/MoS2 interface - providing an additional knob to control the degree of the phase-transition-driven resistivity switching by an external gate voltage. In particular, the commensurate (C) to triclinic (T) phase transition results in an increase in the SBH owing to a collapse of the Mott gap in TaS2. The change in SBH allows us to estimate an electrical Mott gap opening of ~71 +/- 7 meV in the C phase of TaS2. On the other hand, the nearly-commensurate (NC) to incommensurate (IC) phase transition results in a suppression in the SBH, and the heterojunction shows a gate-controlled resistivity switching up to 17.3, which is ~14.5 times higher than that of standalone TaS2. The findings mark an important step forward showing a promising pathway to externally control as well as amplify the CDW induced resistivity switching. This will boost device applications that exploit these phase transitions, such as ultra-broadband photodetection, negative differential conductance, fast oscillator and threshold switching in neuromorphic circuits.",1807.01652v2 2008-10-08,Performance Analysis of 60nm gate length III-V InGaAs HEMTs: Simulations vs. experiments,"An analysis of recent experimental data for high-performance In0.7Ga0.3As high electron mobility transistors (HEMTs) is presented. Using a fully quantum mechanical, ballistic model, we simulate In0.7Ga0.3As HEMTs with gate lengths of LG = 60nm, 85, and 135 nm and compare the result to the measured I-V characteristics including draininduced barrier lowering, sub-threshold swing, and threshold voltage variation with gate insulator thickness, as well as on-current performance. To first order, devices with three different oxide thicknesses and channel lengths can all be described by our ballistic model with appropriate values of parasitic series resistance. For high gate voltages, however, the ballistic simulations consistently overestimate the measured on-current, and they do not show the experimentally observed decrease in on-current with increasing gate length. With no parasitic series resistance at all, the simulated on-current of the LG = 60 nm device is about twice the measured current. According to the simulation, the estimated ballistic carrier injection velocity for this device is about 2.7 x 10^7 cm/s. Because of the importance of the semiconductor capacitance, the simulated gate capacitance is about 2.5 times less than the insulator capacitance. Possible causes of the transconductance degradation observed under high gate voltages in these devices are also explored. In addition to a possible gate-voltage dependent scattering mechanism, the limited ability of the source to supply carriers to the channel, and the effect of nonparabolicity are likely to play a role. The drop in on-current with increasing gate length is an indication that the devices operate below the ballistic limit.",0810.1540v1 2008-12-26,Flux quanta driven by high-density currents in low-impurity V3Si and LuNi2B2C: free flux flow and flux-core size effect,"High density direct currents (DC) are used to drive flux quanta via the Lorentz force towards a highly ordered ""free flux flow"" (FFF) dynamic state, made possible by the weak-pinning environment of high-quality, single-crystal samples of two low-Tc superconducting compounds, V3Si and LuNi2B2C. We report the effect of the magnetic field-dependent fluxon core size on flux flow resistivity rho_f. Much progress has been made in minimizing the technical challenges associated with the use of high currents. Attainment of a FFF phase is indicated by the saturation at highest currents of flux-flow dissipation levels that are well below the normal state resistance and have field-dependent values. The field dependence of the corresponding rho_f is shown to be consistent with a prediction based on a model for the decrease of flux core size at higher fields in weak-coupling BCS s-wave materials.",0812.4715v4 2020-06-01,Radiation hardness of GaAs: Cr and Si sensors irradiated by electron beam,"The interest in using the radiation detectors based on high resistive chromium-compensated GaAs (GaAs:Cr) in high energy physics and others applied fields has been growing steadily due to its numerous advantages over others classical materials. High radiation hardness at room temperature stands out and needs to be systematically investigated. In this paper an experimental study of the effect of 20.9 MeV electrons generated by the LINAC-200 accelerator on some properties of GaAs:Cr based sensors is presented. In parallel, Si sensors were irradiated at the same conditions, measured and analyzed in order to perform a comparative study. The target sensors were irradiated with the dose up to 1.5 MGy. The current-voltage characteristics, resistivity, charge collection efficiency and their dependences on the bias voltage and temperature were measured at different absorbed doses. An analysis of the possible microscopic mechanisms leading to the observed effects in GaAs:Cr sensors is presented in the article.",2006.01254v1 2021-02-04,Quantum Transport in Two-Dimensional WS$_2$ with High-Efficiency Carrier Injection Through Indium Alloy Contacts,"Two-dimensional transition metal dichalcogenides (TMDCs) have properties attractive for optoelectronic and quantum applications. A crucial element for devices is the metal-semiconductor interface. However, high contact resistances have hindered progress. Quantum transport studies are scant as low-quality contacts are intractable at cryogenic temperatures. Here, temperature-dependent transfer length measurements are performed on chemical vapour deposition grown single-layer and bilayer WS$_2$ devices with indium alloy contacts. The devices exhibit low contact resistances and Schottky barrier heights (\sim10 k$\Omega$\si{\micro\metre} at 3 K and 1.7 meV). Efficient carrier injection enables high carrier mobilities ($\sim$190 cm$^2$V$^{-1}$s$^{-1}$) and observation of resonant tunnelling. Density functional theory calculations provide insights into quantum transport and properties of the WS$_2$-indium interface. Our results reveal significant advances towards high-performance WS$_2$ devices using indium alloy contacts.",2102.02489v1 2021-08-11,Single-domain perpendicular magnetization induced by the coherent O 2p-Ru 4d hybridized state in an ultra-high-quality SrRuO3 film,"We investigated the Ru 4d and O 2p electronic structure and magnetic properties of an ultra-high-quality SrRuO3 film on SrTiO3 grown by machine-learning-assisted molecular beam epitaxy. The high itinerancy and long quantum lifetimes of the quasiparticles in the Ru 4d t2g-O 2p hybridized valence band are confirmed by observing the prominent well-screened peak in the Ru 3d core-level photoemission spectrum, the coherent peak near the Fermi energy in the valence band spectrum, and quantum oscillations in the resistivity. The element-specific magnetic properties and the hybridization between the Ru 4d and O 2p orbitals were characterized by Ru M2,3-edge and O K-edge soft X-ray absorption spectroscopy and X-ray magnetic circular dichroism measurements. The ultra-high-quality SrRuO3 film with the residual resistivity ratio of 86 shows the large orbital magnetic moment of oxygen ions induced by the strong orbital hybridization of the O 2p states with the spin-polarized Ru 4d t2g states. The film also shows single-domain perpendicular magnetization with an almost ideal remanent magnetization ratio of 0.97. These results provide detailed insights into the relevance between orbital hybridization and the perpendicular magnetic anisotropy in SrRuO3/SrTiO3 systems.",2108.04980v1 2009-08-03,Resistivity of Mn$_{1-x}$Fe$_x$Si single crystals: Evidence for quantum critical behavior,"Resistivity measurements have been made on Mn$_{1-x}$Fe$_x$Si single crystals between 2 and 300K for $x$ = 0, 0.05, 0.08, 0.12 and 0.15. Fe doping is found to depress the magnetic ordering temperature from 30K for $x$ = 0 to below 2K for $x$ = 0.15. Although Fe doping results in a large increase of the low-temperature residual resistivity, the temperature dependence of the resistivity above the magnetic transition remains practically unaffected by increasing Fe content. An analysis of the temperature derivative of the resistivity provides strong evidence for the existence of a non-Fermi-liquid ground state near $x$ = 0.15 and thus for a quantum critical point tuned by Fe content.",0908.0294v1 2012-10-09,Effect of back-gate on contact resistance and on channel conductance in graphene-based field-effect transistors,"We study the contact resistance and the transfer characteristics of back-gated field effect transistors of mono- and bi-layer graphene. We measure specific contact resistivity of ~7kohm*um2 and ~30kohm*um2 for Ni and Ti, respectively. We show that the contact resistance is a significant contributor to the total source-to-drain resistance and it is modulated by the back-gate voltage. We measure transfer characteristics showing double dip feature that we explain as the effect of doping due to charge transfer from the contacts causing minimum density of states for graphene under the contacts and in the channel at different gate voltage.",1210.2531v1 2013-07-01,Magnetic and transport parameters of LSMO and YBCO/LSMO films deposited on sapphire substrates,"The La0.7Sr0.3MnO3 (LSMO) layers and YBa2Cu3O7-{\delta}/La0.7Sr0.3MnO3 (YBCO/LSMO) bilayers were grown by magnetron sputtering on sapphire (Al2O3 or ALO) substrates. Temperature dependences of resistance of single LSMO films, grown on ALO substrates were typical for polycrystalline manganite materials and the resistance decreased with decrease of the temperature at medium temperatures and increased at lower and higher temperatures. Deposition of a top YBCO layer led to a drastic increase of the sample resistance. These bilayers did not demonstrate a decreasing of the resistance with decrease of temperature. Temperature dependence of the resistance of these samples was interpreted in the framework of a phenomenological model of two intergrain conduction channels. In framework of this model, parameters of the samples were determined and discussed.",1307.0302v1 2015-01-27,Realization of a reversible switching in TaO2 polymorphs via Peierls distortion for resistance random access memory,"Transition-metal-oxide based resistance random access memory is a promising candidate for next-generation universal non-volatile memories. Searching and designing appropriate new materials used in the memories becomes an urgent task. Here, a new structure with the TaO2 formula was predicted using evolutionary algorithms in combination with first-principles calculations. This new structure having a triclinic symmetry (T-TaO2) is both energetically and dynamically more favorable than the commonly believed rutile structure (R-TaO2). Our hybrid functional calculations show that T-TaO2 is a semiconductor with a band gap of 1.0 eV, while R-TaO2 is a metallic conductor. This large difference in electrical property makes TaO2 a potential candidate for resistance random access memory (RRAM). Furthermore, we have shown that T-TaO2 is actually a Peierls distorted R-TaO2 phase and the transition between these two structures is via a directional displacement of Ta atoms. The energy barrier for the reversible phase transition from R-TaO2 to T-TaO2 is 0.19 eV/atom and the other way around is 0.23 eV/atom, suggesting low power consumption for the resistance switch. The present findings provide a new mechanism for the resistance switch and will also stimulate experimental work to fabricate tantalum oxides based RRAM.",1501.06632v1 2015-02-09,Four-Probe Methods for Measuring the Resistivity of Samples in the Form of Rectangular Parallelepipeds,"The problem of measuring the resistivity of isotropic samples of finite dimensions in the form of rectangular parallelepipeds using the four-probe technique was considered. Two variants of contact arrangements were studied: (1) four collinear probes are positioned on one side of a sample symmetrically with respect to the other sides, and (2) two probes on one side of a sample and two on the opposite side are placed precisely in opposite positions and symmetrically with respect to the other sides of the sample (the Schnabel method). Solutions of the problem of the electric field potential distribution in a sample for different positions of the current contacts were found. The solutions were obtained in the form of double series and methods of their summation are presented. The obtained results are extended to the case of measuring the resistivity of anisotropic samples when the resistivity tensor has two independent components. The results of using the developed technique for measuring the resistivity of such a highly anisotropic material as highly oriented pyrolitic graphite using the Schnabel method are presented.",1502.02600v1 2019-12-10,Resistance Drift in Ge2Sb2Te5 Phase Change Memory Line Cells at Low Temperatures and Its Response to Photoexcitation,"Resistance drift in phase change materials is characterized in amorphous phase change memory line-cells from 300 K to 125 K range and is observed to follow the previously reported power-law behavior with drift coefficients in the 0.07 to 0.11 range in dark. While these drift coefficients measured in dark are similar to commonly observed drift coefficients (~0.1) at and above room temperature, measurements under light show a significantly lower drift coefficient (0.05 under illumination versus 0.09 in dark at 150K). Periodic on/off switching of light shows sudden decrease/increase of resistance, attributed to photo-excited carriers, followed by a very slow response (~30 minutes at 150 K) attributed to contribution of charge traps. Continuation of the resistance drift at low temperatures and the observed photo-response suggest that resistance drift in amorphous phase change materials is predominantly an electronic process.",1912.04480v2 2022-04-04,"Inter- to Intra-Layer Resistivity Anisotropy of NdFeAs(O,H) with Various Hydrogen Concentrations","With molecular beam epitaxy and topotactic chemical reaction, we prepared NdFeAs(O,H) epitaxial thin films with various hydrogen concentrations on 5{\deg} vicinal cut MgO substrates. By measuring the resistivities along the longitudinal and transversal directions, the ab plane and the c axis resistivities (\{rho}_ab and \{rho}_c) were obtained. The resistivity anisotropy {\gamma}_\{rho}=\{rho}_c \ \{rho}_ab of NdFeAs(O,H) with various hydrogen concentrations was compared with that of NdFeAs(O,F). At the H concentrations which led to superconducting transition temperatures Tc over 40 K, {\gamma}_\r{ho} recorded ~100-150 at 50 K. On the other hand, a low {\gamma}_\{rho} value of 9 was observed with the mostly doped sample. The exponent \{beta} of the ab plane resistivity obtained by fitting a power law expression \{rho}_{ab}(T)=\{rho}_0+AT^\{beta} to the data was close to unity down to low temperature in the vicinity where the second antiferromagnetic phase locates, which may be related to the quantum critical point discussed at the over-doped side of the phase diagram.",2204.01554v1 2020-04-28,A Route to High-Toughness Battery Electrodes,"There is increasing interest in materials that combine energy-storing functions with augmented mechanical properties, ranging from flexibility in bending to stretchability to structural properties. In the case of lithium-ion batteries, these mechanical functions could enable their integration in emerging technologies such as wearable, free-form electronics and ultimately as structural elements, for example, in transport applications. This work presents a method to produce flexible LiFePO4 LFP electrodes with an extraordinary combination of electrochemical and mechanical performance. Such electrodes exhibit an exceptionally high specific toughness, combined with superior rate capability and energy density, with respect to reference electrodes with typical metallic current collectors. These properties are a result of the strong adhesion of the active material particles to the high surface area carbon nanotube fiber fabric, used as a lightweight, tough, and highly conducting current collector. This strong adherence minimizes electrical resistance, mitigates interfacial failure, and increases ductility through heterogeneous strain after cohesive failure of the inorganic phase. As a result, these electrodes can withstand large deformations before fracture, and, even after fracture, they retain excellent electrochemical performance, approximately double that of unstretched, Al-supported LFP electrodes with equivalent loading.",2004.13350v1 2023-02-02,High-entropy silicide superconductors with W$_{5}$Si$_{3}$-type structure,"We report the synthesis, crystal structure and physical properties of two new high-entropy silicides (HESs), namely (Nb$_{0.1}$Mo$_{0.3}$W$_{0.3}$Re$_{0.2}$Ru$_{0.1}$)$_{5}$Si$_{3}$ and (Nb$_{0.2}$Mo$_{0.3}$W$_{0.3}$Re$_{0.1}$Ru$_{0.1}$)$_{5}$Si$_{3}$. Structural analysis indicates that both HESs consist of a (nearly) single tetragonal W$_{5}$Si$_{3}$-type phase (space group $I$4/$mcm$) with a disordered cation distribution. Electrical resistivity, magnetic susceptibility and specific heat measurements show that (Nb$_{0.1}$Mo$_{0.3}$W$_{0.3}$Re$_{0.2}$Ru$_{0.1}$)$_{5}$Si$_{3}$ and (Nb$_{0.2}$Mo$_{0.3}$W$_{0.3}$Re$_{0.1}$Ru$_{0.1}$)$_{5}$Si$_{3}$ are weakly coupled bulk superconductors, which represent the first superconducting high-entropy nonoxide ceramics. In particular, these HESs have higher $T_{\rm c}$ values (3.2-3.3 K) compared with those of the binary counterparts, and their $B_{\rm c2}$(0)/$T_{\rm c}$ ratios are the largest among superconductors of the same structural type.",2302.00844v1 2024-01-15,Fatigue Behavior of High-Entropy Alloys,"High-entropy alloys (HEAs) refer to alloys composed of five or more elements in equal or near-equal amounts or in an atomic concentration range of 5 to 35 atomic percent (at%). Different elemental ratios will affect the microstructures of HEAs and provide them with unique properties. Based on past research, HEAs have exhibited superior performance, relative to most conventional alloys, with respect to many properties, such as strength, toughness, corrosion resistance, magnetic behavior, etc. Among them, fatigue behavior has been a topic of focus, due to its importance in industrial applications. In this article, we summarized the research progress in the HEA-fatigue behavior in the past ten years, including experimental results and theoretical studies in subdivisions, such as high-cycle fatigue, low-cycle fatigue, fatigue-crack growth, fatigue mechanisms, etc. The influence of the processing and test methods on HEAs is described. The accuracy of several commonly used prediction models is also outlined. Finally, unresolved issues and suggestions on the direction of future research efforts are presented.",2401.07418v1 2024-01-26,Accelerated intermetallic phase amorphization in a Mg-based high-entropy alloy powder,"We describe a novel mechanism for the synthesis of a stable high-entropy alloy powder from an otherwise immiscible Mg-Ti rich metallic mixture by employing high-energy mechanical milling. The presented methodology expedites the synthesis of amorphous alloy powder by strategically injecting entropic disorder through the inclusion of multi-principal elements in the alloy composition. Predictions from first principles and materials theory corroborate the results from microscopic characterizations that reveal a transition of the amorphous phase from a precursor intermetallic structure. This transformation, characterized by the emergence of antisite disorder, lattice expansion, and the presence of nanograin boundaries, signifies a departure from the precursor intermetallic structure. Additionally, this phase transformation is accelerated by the presence of multiple principal elements that induce severe lattice distortion and a higher configurational entropy. The atomic size mismatch of the dissimilar elements present in the alloy produces a stable amorphous phase that resists reverting to an ordered lattice even on annealing.",2401.15197v2 2024-03-28,High Mobility Charge Transport in a Multicarrier Altermagnet CrSb,"A newly identified magnetic phase called altermagnet is being actively studied because of its unprecedented spin-dependent phenomena. Among the candidate materials, CrSb has a particularly high transition temperature and a large spin-splitting energy, but its transport properties have remained unexplored. In this study, we report the magnetotransport properties of CrSb measured on single crystals. We found that the Hall resistivity shows a nonlinear dependence on the magnetic field at low temperatures. From symmetry-based considerations, however, this behavior can not be attributed to an anomalous Hall effect, but to a multicarrier effect. A multicarrier fitting to the in-plane conductivity tensor revealed that there are carriers with high mobilities in CrSb, probably because of the presence of Weyl points in the electronic structure.",2403.19233v1 2014-02-26,MoS2 P-type Transistors and Diodes Enabled by High Workfunction MoOx Contacts,"The development of low-resistance source/drain contacts to transition metal dichalcogenides (TMDCs) is crucial for the realization of high-performance logic components. In particular, efficient hole contacts are required for the fabrication of p-type transistors with MoS2, a model TMDC. Previous studies have shown that the Fermi level of elemental metals is pinned close to the conduction band of MoS2, thus resulting in large Schottky barrier heights for holes with limited hole injection from the contacts. Here, we show that substoichiometric molybdenum trioxide (MoOx, x<3), a high workfunction material, acts as an efficient hole injection layer to MoS2 and WSe2. In particular, we demonstrate MoS2 p-type field-effect transistors and diodes by using MoOx contacts. We also show drastic on-current improvement for p-type WSe2 FETs with MoOx contacts over devices made with Pd contacts, which is the prototypical metal used for hole injection. The work presents an important advance in contact engineering of TMDCs and will enable future exploration of their performance limits and intrinsic transport properties.",1402.6632v1 2015-03-23,Electron-Irradiation Induced Nanocrystallization of Pb(II) in Silica Gels Prepared in High Magnetic Field,"In a previous study, structure of silica gels prepared in a high magnetic field was investigated. While a direct application of such anisotropic silica gels is for an optical anisotropic medium possessing chemical resistance, we show here their possibility of medium in materials processing. In this direction, for example, silica hydrogels have so far been used as media of crystal growth. In this paper, as opposed to the soft-wet state, dried silica gels have been investigated. We have found that lead (II) nanocrystallites were formed induced by electron irradiation to lead (II)-doped dried silica gels prepared in a high magnetic field such as B = 10 T. Hydrogels made from a sodium metasilicate solution doped with lead (II) acetate were prepared. The dried specimens were irradiated by electrons in a transmission electron microscope environment. Electron diffraction patterns indicated the crystallinity of lead (II) nanocrystallites depending on B. An advantage of this processing technique is that the crystallinity can be controlled through the strength of magnetic field B applied during gel preparation. Specific skills are not required to control the strength of magnetic field.",1503.06863v1 2017-04-07,Thermopower and thermal conductivity in the Weyl semimetal NbP,"The Weyl semimetal NbP exhibits an extremely large magnetoresistance (MR) and an ultra-high mobility. The large MR originates from a combination of the nearly perfect compensation between electron- and hole-type charge carriers and the high mobility, which is relevant to the topological band structure. In this work we report on temperature- and field-dependent thermopower and thermal conductivity experiments on NbP. Additionally, we carried out complementary heat capacity, magnetization, and electrical resistivity measurements. We found a giant adiabatic magnetothermopower with a maximum of 800 $\mu$V/K at 50 K in a field of 9 T. Such large effects have been observed rarely in bulk materials. We suggest that the origin of this effect might be related to the high charge-carrier mobility. We further observe pronounced quantum oscillations in both thermal conductivity and thermopower. The obtained frequencies compare well with our heat capacity and magnetization data.",1704.02241v2 2020-10-29,Two-dimensional hole gas in organic semiconductors,"A highly conductive metallic gas that is quantum mechanically confined at a solid-state interface is an ideal platform to explore nontrivial electronic states that are otherwise inaccessible in bulk materials. Although two-dimensional electron gas (2DEG) has been realized in conventional semiconductor interfaces, examples of two-dimensional hole gas (2DHG), which is the counter analogue of 2DEG, are still limited. Here, we report the observation of a 2DHG in solution-processed organic semiconductors in conjunction with an electric double-layer using ionic liquids. A molecularly flat single crystal of high mobility organic semiconductors serves as a defect-free interface that facilitates two-dimensional confinement of high-density holes. Remarkably low sheet resistance of 6 k$\Omega$ and high hole gas density of 10$^{14}$ cm$^{-2}$ result in a metal-insulator transition at ambient pressure. The measured degenerated holes in the organic semiconductors provide a broad opportunity to tailor low-dimensional electronic states using molecularly engineered heterointerfaces.",2010.15883v1 2021-07-29,Synergetic enhancement of power factor and suppression of lattice thermal conductivity via electronic structure modification and nanostructuring on Ni and B co-doped p-type Si-Ge alloy,"For simultaneously achieving the high-power factor and low lattice thermal conductivity of Si-Ge based thermoelectric materials, we employed, in this study, constructively modifying the electronic structure near the chemical potential and nano-structuring by low temperature and high-pressure sintering on nano-crystalline powders. Nickel was doped to create the impurity states near the edge of the valence band for enhancing the power factor with boron for tuning the carrier concentration. The nanostructured samples with the nominal composition of Si0.65-xGe0.32Ni0.03Bx (x = 0.01, 0.02, 0.03, and 0.04) were synthesized by the mechanical alloying followed low-temperature and high-pressure sintering process. A large magnitude of Seebeck coefficient reaching 321 {\mu}VK-1 together with a small electrical resistivity of 4.49 m{\Omega}cm, leads to a large power factor of 2.3 Wm-1K-2 at 1000 K. With successfully reduced thermal conductivity down to 1.47 Wm-1K-1, a large value of ZT ~1.56 was obtained for Si0.65-xGe0.32Ni0.03B0.03 at 1000 K",2107.13778v1 2021-09-03,Growth and characterization of high-quality single-crystalline SnTe retaining cubic symmetry down to the lowest temperature studied,"SnTe, an archetypical topological crystalline insulator, often shows a transition from a highly symmetric cubic phase to a rhombohedral structure at low temperatures. In order to achieve the highly symmetric cubic phase at low temperatures suitable for quantum behaviour, we have employed the modified Bridgman method to grow a high-quality single-crystalline sample of SnTe. Analysis of the crystal structure using Laue diffraction and rocking curve measurements show a very high degree of single crystallinity of the sample. Resistivity and the specific heat data do not show the signature of structural transition down to the lowest temperature studied. The magnetic susceptibility shows diamagnetic behaviour. All these properties manifest the behaviour of a typical bulk semiconductor with conducting surface states as expected in a topological material. Detailed powder x-ray diffraction measurements show cubic structure in the whole temperature range studied.",2109.01420v2 2021-11-22,High-entropy ceramics: propelling applications through disorder,"Disorder enhances desired properties, as well as creating new avenues for synthesizing materials. For instance, hardness and yield stress are improved by solid-solution strengthening, a result of distortions and atomic size mismatches. Thermo-chemical stability is increased by the preference of chemically disordered mixtures for high-symmetry super-lattices. Vibrational thermal conductivity is decreased by force-constant disorder without sacrificing mechanical strength and stiffness. Thus, high-entropy ceramics propel a wide range of applications: from wear resistant coatings and thermal and environmental barriers to catalysts, batteries, thermoelectrics and nuclear energy management. Here, we discuss recent progress of the field, with a particular emphasis on disorder-enhanced properties and applications.",2111.11519v1 2022-11-08,Observation of room-temperature ferroelectricity in elemental Te nanowires,"Ferroelectrics are essential in low-dimensional memory devices for multi-bit storage and high-density integration. A polar structure is a necessary premise for ferroelectricity, mainly existing in compounds. However, it is usually rare in elemental materials, causing a lack of spontaneous electric polarization. Here, we report an unexpected room-temperature ferroelectricity in few-chain Te nanowires. Out-of-plane ferroelectric loops and domain reversal are observed by piezoresponse force microscopy. Through density functional theory, we attribute the ferroelectricity to the ion-displacement created by the interlayer interaction between lone pair electrons. Ferroelectric polarization can induce a strong field effect on the transport along the Te chain, supporting a self-gated field-effect transistor. It enables a nonvolatile memory with high in-plane mobility, zero supply voltage, multilevel resistive states, and a high on/off ratio. Our work provides new opportunities for elemental ferroelectrics with polar structures and paves a way towards applications such as low-power dissipation electronics and computing-in-memory devices.",2211.04066v1 2009-07-17,Study of timing properties of single gap high-resistive bakelite RPC,"The time resolution for several single gap (2 mm) prototype Resistive Plate Chambers (RPC) made of high resistive (bulk resistivity ~ 10^10 - 10^12 ohm cm), 2 mm thick matt finished bakelite paper laminates with silicone coating on the inner surfaces, has been measured. The time resolution for all the modules has been found to be ~ 2 ns at the plateau region.",0907.2982v1 2003-09-16,Metal-insulator transition in EuO,"It is shown that the spectacular metal-insulator transition in Eu-rich EuO can be simulated within an extended Kondo lattice model. The different orders of magnitude of the jump in resistivity in dependence on the concentration of oxygen vacancies as well as the low-temperature resistance minimum in high-resistivity samples are reproduced quantitatively. The huge colossal magnetoresistance (CMR) is calculated and discussed.",0309369v2 2016-08-08,Quantum Criticality and DBI Magneto-resistance,"We use the DBI action from string theory and holography to study the magneto-resistance at quantum criticality with hyperscaling violation. We find and analyze a rich class of scaling behaviors for the magneto-resistance. A special case describes the scaling results found in pnictides by Hayers et al. in~\cite{analytis}.",1608.02598v2 2023-09-19,Resistivity of the two-dimensional Bose-Hubbard model at weak coupling,"We calculate the weak-coupling resistivity of the two-dimensional Bose Hubbard model, comparing with the more familiar fermionic case. At high temperature the resistivity is linear in $T$, while in the low temperature normal state it is exponentially suppressed. We explore the density dependence and calculate the momentum relaxation rate.",2309.10782v1 2018-09-24,Ionic Tuning of Cobaltites at the Nanoscale,"Control of materials through custom design of ionic distributions represents a powerful new approach to develop future technologies ranging from spintronic logic and memory devices to energy storage. Perovskites have shown particular promise for ionic devices due to their high ion mobility and sensitivity to chemical stoichiometry. In this work, we demonstrate a solid-state approach to control of ionic distributions in (La,Sr)CoO$_{3}$ thin films. Depositing a Gd capping layer on the perovskite film, oxygen is controllably extracted from the structure, up-to 0.5 O/u.c. throughout the entire 36 nm thickness. Commensurate with the oxygen extraction, the Co valence state and saturation magnetization show a smooth continuous variation. In contrast, magnetoresistance measurements show no-change in the magnetic anisotropy and a rapid increase in the resistivity over the same range of oxygen stoichiometry. These results suggest significant phase separation, with metallic ferromagnetic regions and oxygen-deficient, insulating, non-ferromagnetic regions, forming percolated networks. Indeed, X-ray diffraction identifies oxygen-vacancy ordering, including transformation to a brownmillerite crystal structure. The unexpected transformation to the brownmillerite phase at ambient temperature is further confirmed by high-resolution scanning transmission electron microscopy which shows significant structural - and correspondingly chemical - phase separation. This work demonstrates room-temperature ionic control of magnetism, electrical resistivity, and crystalline structure in a 36 nm thick film, presenting new opportunities for ionic devices that leverage multiple material functionalities.",1809.08728v1 2020-02-17,Ductile and brittle crack-tip response in equimolar refractory high-entropy alloys,"Understanding the strengthening and deformation mechanisms in refractory high-entropy alloys (HEAs), proposed as new high-temperature material, is required for improving their typically insufficient room-temperature ductility. Here, density-functional theory simulations and a continuum mechanics analysis were conducted to systematically investigate the competition between cleavage decohesion and dislocation emission from a crack tip in the body-centered cubic refractory HEAs HfNbTiZr, MoNbTaVW, MoNbTaW, MoNbTiV, and NbTiVZr. This crack-tip competition is evaluated for tensile loading and a totality of 15 crack configurations and slip systems. Our results predict that dislocation plasticity at the crack tip is generally unfavorable -- although the competition is close for some crack orientations, suggesting intrinsic brittleness and low crack-tip fracture toughness in these five HEAs at zero temperature. Fluctuations in local alloy composition, investigated for HfNbTiZr, can locally reduce the resistance to dislocation emission for a slip system relative to the configuration average of that slip system, but do not change the dominant crack-tip response. In the case of single-crystal MoNbTaW, where an experimental, room-temperature fracture-toughness value is available for a crack on a \{100\} plane, theoretical and experimental results agree favorably. Factors that may limit the agreement are discussed. We survey the effect of material anisotropy on preferred crack tip orientations, which are found to be alloy specific. Mixed-mode loadings are found to shift the competition in favor of cleavage or dislocation nucleation, depending on crack configuration and amplified by the effect of material anisotropy on crack tip stresses.",2002.07013v1 2019-08-22,Non-localized states and high hole mobility in amorphous germanium,"Covalent amorphous semiconductors, such as amorphous silicon (a-Si) and germanium (a-Ge), are commonly believed to have localized electronic states at the top of the valence band and the bottom of the conduction band. Electrical conductivity is thought to be by the hopping mechanism through localized states. The carrier mobility of these materials is usually very low, in the order of ~10^-3 - 10^-2 cm^2/(Vs) at room temperature. In this study, we present the Hall effect characterization of a-Ge prepared by self-ion implantation of Ge ions. The a-Ge prepared by this method is highly homogenous and has a mass density within 98.5% of the crystalline Ge. The material exhibits an exceptionally high electrical conductivity and carrier mobility (~100 cm^2/(Vs)) for an amorphous semiconductor. The temperature-dependent resistivity of the material is very-well defined with two distinctive regions, extrinsic and intrinsic conductivity, as in crystalline Ge. These results are direct evidence for a largely-preserved band structure and non-localized states of the valence band in a-Ge, as proposed by Tauc et al. from optical characterization alone. This finding is not only significant for the understanding of electrical conductivity in covalent disordered semiconductors, but the exceptionally high mobility we have observed in amorphous Ge opens up device applications not previously considered for amorphous semiconductors.",1908.08246v1 2020-11-20,StressNet: Deep Learning to Predict Stress With Fracture Propagation in Brittle Materials,"Catastrophic failure in brittle materials is often due to the rapid growth and coalescence of cracks aided by high internal stresses. Hence, accurate prediction of maximum internal stress is critical to predicting time to failure and improving the fracture resistance and reliability of materials. Existing high-fidelity methods, such as the Finite-Discrete Element Model (FDEM), are limited by their high computational cost. Therefore, to reduce computational cost while preserving accuracy, a novel deep learning model, ""StressNet,"" is proposed to predict the entire sequence of maximum internal stress based on fracture propagation and the initial stress data. More specifically, the Temporal Independent Convolutional Neural Network (TI-CNN) is designed to capture the spatial features of fractures like fracture path and spall regions, and the Bidirectional Long Short-term Memory (Bi-LSTM) Network is adapted to capture the temporal features. By fusing these features, the evolution in time of the maximum internal stress can be accurately predicted. Moreover, an adaptive loss function is designed by dynamically integrating the Mean Squared Error (MSE) and the Mean Absolute Percentage Error (MAPE), to reflect the fluctuations in maximum internal stress. After training, the proposed model is able to compute accurate multi-step predictions of maximum internal stress in approximately 20 seconds, as compared to the FDEM run time of 4 hours, with an average MAPE of 2% relative to test data.",2011.10227v1 2022-05-16,Single Crystalline 2D Material Nanoribbon Networks for Nanoelectronics,"The last decade has seen a flurry of studies related to graphene nanoribbons owing to their potential applications in the quantum realm. However, little experimental work has been reported towards nanoribbons of other 2D materials due to the absence of synthesis routes. Here, we propose a universal approach to synthesize high-quality networks of nanoribbons from arbitrary 2D materials while maintaining high crystallinity, sufficient yield, narrow size distribution, and straight-forward device integrability. The wide applicability of this technique is demonstrated by fabricating MoS2, WS2, WSe2, and graphene nanoribbon field effect transistors that inherently do not suffer from interconnection resistances. By relying on self-assembled and self-aligned organic nanostructures as masks, we demonstrate the possibility of controlling the predominant crystallographic direction of the nanoribbon's edges. Electrical characterization shows record mobilities and very high ON currents for various TMDCs despite extreme width scaling. Lastly, we explore decoration of nanoribbon edges with plasmonic particles paving the way towards the development of nanoribbon-based plasmonic sensing and opto-electronic devices.",2205.09507v1 2023-04-18,Controllable Strain-driven Topological Phase Transition and Dominant Surface State Transport in High-Quality HfTe5 Samples,"Controlling materials to create and tune topological phases of matter could potentially be used to explore new phases of topological quantum matter and to create novel devices where the carriers are topologically protected. It has been demonstrated that a trivial insulator can be converted into a topological state by modulating the spin-orbit interaction or the crystal lattice. However, there are limited methods to controllably and efficiently tune the crystal lattice and at the same time perform electronic measurements at cryogenic temperatures. Here, we use large controllable strain to demonstrate the topological phase transition from a weak topological insulator phase to a strong topological insulator phase in high-quality HfTe5 samples. After applying high strain to HfTe5 and converting it into a strong topological insulator, we found that the sample's resistivity increased by more than two orders of magnitude (24,000%) and that the electronic transport is dominated by the topological surface states at cryogenic temperatures. Our findings show that HfTe5 is an ideal material for engineering topological properties, and it could be generalized to study topological phase transitions in van der Waals materials and heterostructures. These results can pave the way to create novel devices with applications ranging from spintronics to fault-tolerant topologically protected quantum computers.",2304.09072v1 2016-12-17,Electric Properties of Dirac Fermions Captured into 3D Nanoporous Graphene Networks,"Graphene, as a promising material of post-silicon electronics, opens a new paradigm for the novel electronic properties and device applications. On the other hand, the 2D feature of graphene makes it technically challenging to be integrated into 3D transistors with a sufficient processor capacity. Although there are many attempts to assemble 2D graphene into 3D structures, the characteristics of massless Dirac fermions cannot be well preserved in these materials for transistor applications. Here we report a high-performance graphene transistor by utilizing 3D nanoporous graphene which is comprised of an interconnected single graphene sheet and a commodious open porosity to infuse an ionic liquid for a tunable electronic state by applying electric fields. The 3D nanoporous graphene transistor, with high carrier mobility of 5000-7500 cm$^2$V$^{-1}$s$^{-1}$, exhibits two to three orders of magnitude higher electric conductance and capacitance than those of 2D graphene devices, along with preserved ambipolor electronic nature of Dirac cones. Moreover, the 3D graphene networks with Dirac fermions turn out to exhibit a unique nonlinear Hall resistance in a wide range of the gate voltages. The high quality 3D nanoporous graphene EDLT may open a new field for utilizing Dirac fermions in 3D network structures for various fundamental and practical applications.",1612.05716v1 2017-11-24,Stability of Thin Film Refractory Plasmonic Materials Taken to High Temperatures in Air,"Materials such as W, TiN, and SrRuO3 (SRO) have been suggested as promising alternatives to Au and Ag in plasmonic applications owing to their refractory properties. However, investigation of the reproducibility of the optical properties after thermal cycling at high operational temperatures is so far lacking. Here, thin films of W, Mo, Ti, TiN, TiON, Ag, Au, and SrRuO3 are investigated to assess their viability for robust refractory plasmonic applications. Films ranging in thickness from 50 - 180 nm are deposited on MgO and Si substrates by RF magnetron sputtering and, in the case of SrRuO3, pulsed laser deposition, prior to characterisation by means of AFM, XRD, spectroscopic ellipsometry, and DC resistivity. Measurements are conducted before and after annealing in air at temperatures ranging from 300 - 1000{\deg} C for one hour, to establish the maximum cycling temperature and potential longevity at temperature for each material. It is found that SrRuO3 retains metallic behaviour after annealing at 800{\deg} C, however, importantly, the optical properties of TiN and TiON are degraded as a result of oxidation. Nevertheless, both TiN and TiON may be better suited than Au or SRO for high temperature applications operating under vacuum conditions.",1711.08923v1 2016-03-17,Transport evidence for the three-dimensional Dirac semimetal phase in ZrTe5,"Topological Dirac semimetal is a newly discovered class of materials and has attracted intense attentions. This material can be viewed as a three-dimensional (3D) analogue of graphene and has linear energy dispersion in bulk, leading to a range of exotic transport properties. Here we report direct quantum transport evidence of 3D Dirac semimetal phase of layered material ZrTe5 by angular dependent magnetoresistance measurements under high magnetic fields up to 31 Tesla. We observed very clear negative longitudinal magnetoresistance induced by chiral anomaly under the condition of the magnetic field aligned only along the current direction. Pronounced Shubnikov-de Hass (SdH) quantum oscillations in both longitudinal magnetoresistance and transverse Hall resistance were observed, revealing anisotropic light cyclotron masses and high mobility of the system. In particular, a nontrivial {\pi}-Berry phase in the SdH gives clear evidence for 3D Dirac semimetal phase. Furthermore, we observed clear Landau Level splitting under high magnetic field, suggesting possible splitting of Dirac point into Weyl points due to broken time reversal symmetry. Our results indicate that ZrTe5 is an ideal platform to study 3D massless Dirac and Weyl fermions in a layered compound.",1603.05351v2 2022-06-16,Scalable Composites Benefiting from Transition-Metal Oxides as Cathode Materials for Efficient Lithium-Sulfur Batteries,"Composite materials achieved by including transition-metal oxides with different structures and morphologies in sulfur are suggested as scalable cathodes for high-energy lithium-sulfur (Li-S) batteries. The composites contain 80 wt.% sulfur and 20 wt.% of either MnO2 or TiO2, leading to a sulfur content in the electrode of 64 wt.% and revealing a reversible, fast, and lowly polarized conversion process in the cell with limited interphase resistance. The S-TiO2 composite exhibits an excellent rate capability between C/10 and 2C, and a cycle life extended over 400 cycles at 2C, owing to the effects of the nanometric TiO2 additive in boosting the reaction kinetics. Instead, the micrometric sized particles of MnO2 partially limit the electrochemical activity of S-MnO2 to the current rate of 1C. Nevertheless, both S-MnO2 and S-TiO2 withstand a sulfur loading up to values approaching 6 mgcm-2, and deliver an areal capacit ranging from about 4.5 to 5.5 mAhcm-2 at C/5. The excellent performances of the metal oxide-sulfur electrodes, even at high active material loading, and the possible scalability of the synthetic pathway adopted in the work suggest that the composites are viable cathodes for next-generation Li-S batteries with high energy density and efficient electrochemical process.",2206.14569v1 2024-01-25,Spatially Resolved High Voltage Kelvin Probe Force Microcopy: A Novel Avenue for Examining Electrical Phenomena at Nanoscale,"Kelvin probe microscopy (KPFM) is a well-established scanning probe technique, used to measure surface potential accurately; it has found extensive use in the study of a range of materials phenomena. In its conventional form, KPFM frustratingly precludes imaging samples or scenarios where large surface potential exists or large surface potential gradients are created outside the typical +/-10V window. If the potential regime measurable via KPFM could be expanded, to enable precise and reliable metrology, through a high voltage KPFM (HV-KPFM) adaptation, it could open up pathways towards a range of novel experiments, where the detection limit of regular KPFM has so far prevented the use of the technique. In this work, HV-KPFM has been realised and shown to be capable of measuring large surface potential and potential gradients with accuracy and precision. The technique has been employed to study a range of materials (positive temperature coefficient of resistivity ceramics, charge storage fluoropolymers and pyroelectrics) where accurate spatially resolved mapping of surface potential within high voltage regime facilitates novel physical insight. The results demonstrate that HV-KPFM can be used as an effective tool to fill in existing gaps in surface potential measurements while also opening routes for novel studies in materials physics.",2401.14124v1 2024-02-05,High Strain Engineering of a Suspended WSSe Monolayer Membrane by Indentation and Measured by Tip-enhanced Photoluminescence,"Straintronics involves the manipulation and regulation of the electronic characteristics of 2D materials through the use of macro- and nano-scale strain engineering. In this study, we utilized an atomic force microscope (AFM) coupled with an optical system to perform indentation measurements and tip-enhanced photoluminescence (TEPL), allowing us to extract the local optical response of a suspended monolayer membrane of ternary WSSe at various levels of deformation, up to strains of 10%. The photoluminescence signal is modelled considering the deformation, stress distribution and strain dependence of the WSSe band structure. We observe an additional TEPL signal that exhibits significant variation under strain, with 64 meV per percent of elongation. This peak is linked to the highly strained 2D material lying right underneath the tip. We discuss the amplification of the signal and its relation to the excitonic funnelling effect in a more comprehensive model. We will also compare the diffusion caused by Auger recombination against the radiative excitonic decay. We use TEPL to examine and comprehend the local physics of 2D semi-conducting materials subjected to extreme mechanical strain. Chemical vapour deposition-fabricated 2D ternaries possess high strain resistance, comparable to the benchmark MoS2, and a high Young's modulus of 273 GPa.",2402.03061v1 2019-08-11,Magnetotransport as diagnostic of spin reorientation: kagome ferromagnet as a case study,"While in most ferro or antiferromagnetic materials there is a unique crystallographic direction, including crystallographically equivalent directions, in which the moments like to point due to spin-orbit coupling, in some, the direction of the spin reorients as a function of a certain physical parameter such as temperature, pressure etc. Fe3Sn2 is a kagome ferromagnet with an onset of ferromagnetism below 650 K, and undergoes a spin reorientation near 150 K. While it is known that the moments in Fe3Sn2 point perpendicular to the kagome plane at high temperatures and parallel to the kagome plane at low temperatures, how the distribution of the magnetic domains in the two different spin orientations evolve throughout the spin reorientation is not well known. Furthermore, while there have been various reports on the magnetotransport properties in the Hall configuration, the angular dependence of magnetoresistance has not been studied so far. In this paper, we have examined the spin reorientation by using anisotropic magnetoresistivity in detail, exploiting the dependence of the resistivity on the direction between magnetization and applied current. We are able to determine the distribution of the magnetic domains as a function of temperature between 360 K to 2 K and the reorientation transition to peak at 120 K. We discover that both out of plane and in plane phases coexist at temperatures around the spin reorientation, indicative of a first order transition. Although the volume of the magnetic domains in the different phases sharply changes at the spin reorientation transition, the electronic structure for a specific magnetization is not influenced by the spin reorientation. In contrast, we observe an electronic transition around 40 K, hitherto unreported, and reflected in both the zero-field resistivity and anisotropic resistivity.",1908.03927v1 2021-11-22,Shape-Dependent Multi-Weight Magnetic Artificial Synapses for Neuromorphic Computing,"In neuromorphic computing, artificial synapses provide a multi-weight conductance state that is set based on inputs from neurons, analogous to the brain. Additional properties of the synapse beyond multiple weights can be needed, and can depend on the application, requiring the need for generating different synapse behaviors from the same materials. Here, we measure artificial synapses based on magnetic materials that use a magnetic tunnel junction and a magnetic domain wall. By fabricating lithographic notches in a domain wall track underneath a single magnetic tunnel junction, we achieve 4-5 stable resistance states that can be repeatably controlled electrically using spin orbit torque. We analyze the effect of geometry on the synapse behavior, showing that a trapezoidal device has asymmetric weight updates with high controllability, while a straight device has higher stochasticity, but with stable resistance levels. The device data is input into neuromorphic computing simulators to show the usefulness of application-specific synaptic functions. Implementing an artificial neural network applied on streamed Fashion-MNIST data, we show that the trapezoidal magnetic synapse can be used as a metaplastic function for efficient online learning. Implementing a convolutional neural network for CIFAR-100 image recognition, we show that the straight magnetic synapse achieves near-ideal inference accuracy, due to the stability of its resistance levels. This work shows multi-weight magnetic synapses are a feasible technology for neuromorphic computing and provides design guidelines for emerging artificial synapse technologies.",2111.11516v2 2014-11-04,Tackling drug resistant infection outbreaks of global pandemic Escherichia coli ST131 using evolutionary and epidemiological genomics,"High-throughput molecular screening is required to investigate the origin and diffusion of antimicrobial resistance in pathogen outbreaks. The most frequent cause of human infection is Escherichia coli, which is dominated by sequence type 131 (ST131), a set of rapidly radiating pandemic clones. The highly infectious clades of ST131 originated firstly by a mutation enhancing virulence and adhesion. Secondly, single-nucleotide polymorphisms occurred enabling fluoroquinolone-resistance, which is near-fixed in all ST131. Thirdly, broader resistance through beta-lactamases has been gained and lost frequently, symptomatic of conflicting environmental selective effects. This flexible approach to gene exchange is worrying and supports the proposition that ST131 will develop an even wider range of plasmid and chromosomal elements promoting antimicrobial resistance. To stymie ST131, deep genome sequencing is required to understand the origin, evolution and spread of antimicrobial resistance genes. Phylogenetic methods that decipher past events can predict future patterns of virulence and transmission based on genetic signatures of adaptation and gene exchange. Both the effect of partial antimicrobial exposure and cell dormancy caused by variation in gene expression may accelerate the development of resistance. High-throughput sequencing can decode measurable evolution of cell populations within patients associated with systems-wide changes in gene expression during treatments. A multi-faceted approach can enhance assessment of antimicrobial resistance in E. coli ST131 by examining transmission dynamics between hosts to achieve a goal of pre-empting resistance before it emerges by optimising antimicrobial treatment protocols.",1411.0905v3 2014-09-25,Recycled nylon fibers as cement mortar reinforcement,"We investigate engineering applications of recycled nylon fibers obtained from waste fishing nets, focusing our attention on the use of recycled nylon fibers as tensile reinforcement of cementitious mortars. We begin by characterizing the tensile behavior of both unconditioned and alkali-cured recycled nylon fibers obtained through manual cutting of waste fishing net filaments, with the aim of assessing the resistance of such materials to chemical attacks. Special attention is also given to evaluating the workability of fresh mortar and the possible impacts of contaminants released by waste fishing nets into the environment. Next, we deal with compression and bending tests on cementitious mortars reinforced with recycled nylon fibers, and establish comparisons with the experimental behavior of the unreinforced material and with results given in existing literature. In our analysis of different weight fractions and aspect ratios of the reinforcing fibers, we observe marked increases in the tensile strength (up to +35%) and toughness (up to 13 times greater) of the nylon reinforced mortar, as compared with the unreinforced material. The presented results emphasize the high environmental and mechanical potential of recycled nylon fibers for the reinforcement of sustainable cement mortars.",1409.7258v4 2019-05-14,Ohmic contact engineering in few-layer black Phosphorus field effect transistors,"Achieving good quality Ohmic contacts to van der Waals materials is a challenge, since at the interface between metal and van der Waals material, different conditions can occur, ranging from the presence of a large energy barrier between the two materials to the metallization of the layered material below the contacts. In black phosphorus (bP), a further challenge is its high reactivity to oxygen and moisture, since the presence of uncontrolled oxidation can substantially change the behavior of the contacts. In this study, we investigate the influence of the metal used for the contacts to bP against the variability between different flakes and different samples, using three of the most used metals as contacts: Chromium, Titanium, and Nickel. Using the transfer length method, from an analysis of ten devices, both at room temperature and at low temperature, Ni results to be the best metal for Ohmic contacts to bP, providing the lowest contact resistance and minimum scattering between different devices. Moreover, we investigate the gate dependence of the current-voltage characteristics of these devices. In the accumulation regime, we observe good linearity for all metals investigated.",1905.05649v1 2019-06-24,Conductivity of Dirac-like surface states in correlated honeycomb transition metal oxide Mott insulators,"The search for materials with novel and unusual electronic properties is at the heart of condensed matter physics as well as the basis to develop conceptual new technologies. In this context, the correlated honeycomb transition metal oxides attract large attention for both, being a possible experimental realization of the theoretically predicted magnetic Kitaev exchange and the theoretical prospect of topological nontriviality. The Mott insulating sodium iridate is prototypical among these materials with the promising prospect to bridge the field of strongly correlated systems with topology, finally opening a path to a wide band gap material with exotic surface properties. Here, we report a profound study of the electronic properties of ultra-high-vacuum cleaved surfaces combining transport measurements with scanning tunneling techniques, showing that multiple conductive channels with differing nature are simultaneously apparent in this material. Most importantly, a V-shaped density of states and a low sheet resistance, in spite of a large defect concentration, point towards a topologically protected surface conductivity contribution. By incorporating the issue of the addressability of electronic states in the tunneling process, we develop a framework connecting previous experimental results as well as theoretical considerations.",1906.09809v2 2020-07-22,Impact of Li$_{2.9}$B$_{0.9}$S$_{0.1}$O$_{3.1}$ glass additive on the structure and electrical properties of the LATP-based ceramics,"The existing solid electrolytes for lithium ion batteries suffer from low total ionic conductivity, which restricts its usefulness for the lithium-ion battery technology. Among them, the NASICON-based materials, such as Li1.3Al0.3Ti1.7(PO4)3 (LATP) exhibit low total ionic conductivity due to highly resistant grain boundary phase. One of the possible approaches to efficiently enhance their total ionic conductivity is the formation of a composite material. Herein, the Li2.9B0.9S0.1O3.1 glass, called LBSO hereafter, was chosen as an additive material to improve the ionic properties of the ceramic Li1.3Al0.3Ti1.7(PO4)3 base material. The properties of this Li1.3Al0.3Ti1.7(PO4)3-xLi2.9B0.9S0.1O3.1 (0 < x < 0.3) system have been studied by means of high temperature X-ray diffractometry (HTXRD), 7Li, 11B, 27Al and 31P magic angle spinning nuclear magnetic resonance spectroscopy (MAS NMR), thermogravimetry (TG), scanning electron microscopy (SEM), impedance spectroscopy (IS) and density methods. We show here that the introduction of the foreign LBSO phase enhances their electric properties. This study reveals several interesting correlations between the apparent density, the microstructure, the composition, the sintering temperature and the ionic conductivity. Moreover, the electrical properties of the composites will be discussed in the terms of the brick-layer model (BLM). The highest value of {\sigma}tot = 1.5 x 10-4 Scm-1 has been obtained for LATP-0.1LBSO material sintered at 800{\deg}C.",2007.11244v2 2020-12-16,Anisotropic phonon-mediated electronic transport in chiral Weyl semimetals,"Discovery and observations of exotic, quantized optical and electrical responses have sparked renewed interest in nonmagnetic chiral crystals. Within this class of materials, six group V transition metal ditetrelides, that is, XY$_2$ (X = V, Nb, Ta and Y = Si, Ge), host composite Weyl nodes on high-symmetry lines, with Kramers-Weyl fermions at time-reversal invariant momenta. In addition, at least two of these materials, NbGe$_2$ and NbSi$_2$, exhibit superconducting transitions at low temperatures. The interplay of strong electron-phonon interaction and complex Fermi surface topology present an opportunity to study both superconductivity and hydrodynamic electron transport in these systems. Towards this broader question, we present an ab initio theoretical study of the electronic transport and electron-phonon scattering in this family of materials, with a particular focus on NbGe$_2$ vs. NbSi$_2$, and the other group V ditetrelides. We shed light on the microscopic origin of NbGe$_2$'s large and anisotropic room temperature resistivity and contextualize its strong electron-phonon scattering with a presentation of other relevant scattering lifetimes, both momentum-relaxing and momentum-conserving. Our work explores the intriguing possibility of observing hydrodynamic electron transport in these chiral Weyl semimetals.",2012.09207v1 2022-08-15,Valley-coherent quantum anomalous Hall state in AB-stacked MoTe2/WSe2 bilayers,"Moir\'e materials provide fertile ground for the correlated and topological quantum phenomena. Among them, the quantum anomalous Hall (QAH) effect, in which the Hall resistance is quantized even under zero magnetic field, is a direct manifestation of the intrinsic topological properties of a material and an appealing attribute for low-power electronics applications. The QAH effect has been observed in both graphene and transition metal dichalcogenide (TMD) moir\'e materials. It is thought to arise from the interaction-driven valley polarization of the narrow moir\'e bands. Here, we show surprisingly that the newly discovered QAH state in AB-stacked MoTe2/WSe2 moir\'e bilayers is not valley-polarized but valley-coherent. The layer- and helicity-resolved optical spectroscopy measurement reveals that the QAH ground state possesses spontaneous spin (valley) polarization aligned (anti-aligned) in two TMD layers. In addition, saturation of the out-of-plane spin polarization in both layers occurs only under high magnetic fields, supporting a canted spin texture. Our results call for a new mechanism for the QAH effect and highlight the potential of TMD moir\'e materials with strong electronic correlations and spin-orbit interactions for exotic topological states.",2208.07452v1 2022-09-26,Evaluating Effects of Geometry and Material Composition on Production of Transversely Shaped Beams from Diamond Field Emission Array Cathodes,"Field emission cathodes (FECs) are attractive for the next generation of injectors due to their ability to provide high current density bright beams with low intrinsic emittance. One application of FECs worthy of special attention is to provide transversely shaped electron beams for emittance exchange that translates a transverse electron beam pattern into a longitudinal pattern. FECs can be fabricated in a desired pattern and produce transversely shaped beams without the need for complex masking or laser schemes. However, reliable and consistent production of transversely shaped beams is affected by material properties of the FEC. This paper reports the results of testing two diamond field emitter array (DFEA) FECs with the same lithography pattern and emitter geometry but different material and tip characteristics. Although both cathodes were able to sustain gradients of 44 MV/m and produce maximum output integral charge of 0.5 nC per radiofrequency (rf) pulse, their emission patterns were quite different. One cathode did not produce a patterned beam while the other one did. Differences in field emission characteristics and patterned beam production were explained by the differences in the tip geometry and the cathode material properties. The main practical takeaway was found to be that the tip sharpness was not a prerequisite for good patterned beam production. Instead, other material characteristics, such as the ballast resistance, determined cathode performance.",2209.13047v1 2023-04-13,Effect of hirtisation on the roughness and fatigue performance of porous titanium lattice structures,"Additive manufacturing (AM) has enabled the fabrication of extremely complex components such as porous metallic lattices, which have applications in aerospace, automotive, and in particular biomedical devices. The fatigue resistance of these materials is currently an important limitation however, due to manufacturing defects such as semi-fused particles and weld lines. Here Hirtisation$^\circledR$ is used for post-processing of Ti-6Al-4V lattices, reducing the strut surface roughness (Sa) from 12 to 6 $\mu$m, removing all visible semi-fused particles. The evenness of this treatment in lattices with $\rho /\rho_{s}$ up to 18.3% and treatment depth of 6.5 mm was assessed, finding no evidence of reduced effectiveness on internal surfaces. After normalising to quasi-static mechanical properties to account for material losses during hirtisation (34-37% reduction in strut diameter), the fatigue properties show a marked improvement due to the reduction in surface roughness. Normalised high cycle fatigue strength ($\sigma_{f,10^{6}}/\sigma_{y}$) increased from around 0.1 to 0.16-0.21 after hirtisation, an average increase of 80%. For orthopaedic implant devices where matching the stiffness of surrounding bone is crucial, the $\sigma_{f}/E$ ratio is a key metric. After hirtisation the $\sigma_{f}/E$ ratio increased by 90%, enabling design of stiffness matched implant materials with greater fatigue strength. This work demonstrates that hirtisation is an effective method for improving the surface roughness of porous lattice materials, thereby enhancing their fatigue performance.",2304.06621v1 2024-03-15,An inflated dynamic Laplacian to track the emergence and disappearance of semi-material coherent sets,"Lagrangian methods continue to stand at the forefront of the analysis of time-dependent dynamical systems. Most Lagrangian methods have criteria that must be fulfilled by trajectories as they are followed throughout a given finite flow duration. This key strength of Lagrangian methods can also be a limitation in more complex evolving environments. It places a high importance on selecting a time window that produces useful results, and these results may vary significantly with changes in the flow duration. We show how to overcome this drawback in the tracking of coherent flow features. Finite-time coherent sets (FTCS) are material objects that strongly resist mixing in complicated nonlinear flows. Like other materially coherent objects, by definition they must retain their coherence properties throughout the specified flow duration. Recent work [Froyland and Koltai, CPAM, 2023] introduced the notion of semi-material FTCS, whereby a balance is struck between the material nature and the coherence properties of FTCS. This balance provides the flexibility for FTCS to come and go, merge and separate, or undergo other changes as the governing unsteady flow experiences dramatic shifts. The purpose of this work is to illustrate the utility of the inflated dynamic Laplacian introduced in [Froyland and Koltai, CPAM, 2023] in a range of dynamical systems that are challenging to analyse by standard Lagrangian means, and to provide an efficient meshfree numerical approach for the discretisation of the inflated dynamic Laplacian.",2403.10360v1 2024-03-20,Tailoring Physical Properties of Crystals through Synthetic Temperature Control: A Case Study for new Polymorphic NbFeTe2 phases,"Growth parameters play a significant role in the crystal quality and physical properties of layered materials. Here we present a case study on a van der Waals magnetic NbFeTe2 material. Two different types of polymorphic NbFeTe2 phases, synthesized at different temperatures, display significantly different behaviors in crystal symmetry, electronic structure, electrical transport, and magnetism. While the phase synthesized at low temperature showing behavior consistent with previous reports, the new phase synthesized at high temperature, has completely different physical properties, such as metallic resistivity, long-range ferromagnetic order, anomalous Hall effect, negative magnetoresistance, and distinct electronic structures. Neutron diffraction reveals out-of-plane ferromagnetism below 70K, consistent with the electrical transport and magnetic susceptibility studies. Our work suggests that simply tuning synthetic parameters in a controlled manner could be an effective route to alter the physical properties of existing materials potentially unlocking new states of matter, or even discovering new materials.",2403.13596v1 2022-07-06,Proposal for semiconductor-free negative differential resistance tunnel diode with ultra-high peak-to-valley current ratio,"The negative differential resistance (NDR) tunnel diodes are promising alternative devices for beyond-CMOS computing as they offer several potential applications when integrated with transistors. We propose a novel semiconductor-free NDR tunnel diode concept that exhibits an ultra-high peak-to-valley current ratio (PVCR) value. Our proposed NDR diode consists of two cold metal electrodes separated by a thin insulating tunnel barrier. The NDR effect stems from the unique electronic band structure of the cold metal electrodes, i.e., the width of the isolated metallic bands around the Fermi level as well as the energy gaps separating higher- and lower-lying bands determine the current-voltage ($I$-$V$) characteristics and the PVCR value of the tunnel diode. By proper choice of the cold metal electrode materials, either a conventional N-type or ${\Lambda}$-type NDR effect can be obtained. Two-dimensional (2D) materials offer a unique platform for the realization of proposed NDR tunnel diodes. To demonstrate the proof of concept we employ the nonequilibrium Green function method combined with density functional theory to calculate the $I$-$V$ characteristic of the lateral (AlI$_2$/MgI$_2$/AlI$_2$) and vertical (NbS$_2$/h-BN/NbS$_2$) heterojunction tunnel diodes based on 2D cold metals. For the lateral tunnel diode, we obtain a ${\Lambda}$-type NDR effect with an ultra-high PVCR value of 10$^{16}$ at room temperature, while the vertical tunnel diode exhibits a conventional N-type NDR effect with a smaller PVCR value of about 10$^4$. The proposed concept provides a semiconductor-free solution for NDR devices to achieve desired $I$-$V$ characteristics with ultra-high PVCR values for memory and logic applications.",2207.02593v2 2001-02-12,Temperature- and magnetic-field-dependent resistivity of MgB2 sintered at high temperature and high pressure condition,"We report the temperature- and magnetic-field-dependent resistivity of MgB2 sintered at high temperature and high pressure condition. The superconducting transition width for the resistivity measurement was about 0.4 K, and the low-field magnetization showed a sharp superconducting transition with a transition width of about 1 K. The resistivity in the normal state roughly followed T^2 behavior with smaller residual resistivity ratio (RRR) of 3 over broad temperature region above 100 K rather than reported T^3 behavior with larger RRR value of ~ 20 in the samples made at lower pressures. Also, the resistivity did not change appreciably with the applied magnetic field, which was different from previous report. These differences were discussed with the microscopic and structural change due to the high-pressure sintering.",0102215v4 2017-03-01,Size Dependence of Nanoscale Wear of Silicon Carbide,"Nanoscale, single-asperity wear of single-crystal silicon carbide (sc-SiC) and nanocrystalline silicon carbide (nc-SiC) is investigated using single-crystal diamond nanoindenter tips and nanocrystalline diamond atomic force microscopy (AFM) tips under dry conditions, and the wear behavior is compared to that of single-crystal silicon with both thin and thick native oxide layers. We discovered a transition in the relative wear resistance of the SiC samples compared to that of Si as a function of contact size. With larger nanoindenter tips (tip radius around 370 nm), the wear resistances of both sc-SiC and nc-SiC are higher than that of Si. This result is expected from the Archard's equation because SiC is harder than Si. However, with the smaller AFM tips (tip radius around 20 nm), the wear resistances of sc-SiC and nc-SiC are lower than that of Si, despite the fact that the contact pressures are comparable to those applied with the nanoindenter tips, and the plastic zones are well-developed in both sets of wear experiments. We attribute the decrease in the relative wear resistance of SiC compared to that of Si to a transition from a wear regime dominated by the materials' resistance to plastic deformation (i.e., hardness) to a regime dominated by the materials' resistance to interfacial shear. This conclusion is supported by our AFM studies of wearless friction, which reveal that the interfacial shear strength of SiC is higher than that of Si. The contributions of surface roughness and surface chemistry to differences in interfacial shear strength are also discussed.",1703.01181v1 2022-02-09,Scalable $\rm Al_2O_3-TiO_2$ Conductive Oxide Interfaces as Defect Reservoirs for Resistive Switching Devices,"Resistive switching devices herald a transformative technology for memory and computation, offering considerable advantages in performance and energy efficiency. Here we employ a simple and scalable material system of conductive oxide interfaces and leverage their unique properties for a new type of resistive switching device. For the first time, we demonstrate an $\rm Al_2O_3-TiO_2$ based valence-change resistive switching device, where the conductive oxide interface serves both as the back electrode and as a reservoir of defects for switching. The amorphous-polycrystalline $\rm Al_2O_3-TiO_2$ conductive interface is obtained following the technological path of simplifying the fabrication of the two-dimensional electron gases (2DEGs), making them more scalable for practical mass integration. We combine physical analysis of the device chemistry and microstructure with comprehensive electrical analysis of its switching behavior and performance. We pinpoint the origin of the resistive switching to the conductive oxide interface, which serves as the bottom electrode and as a reservoir of oxygen vacancies. The latter plays a key role in valence-change resistive switching devices. The new device, based on scalable and complementary metal-oxide-semiconductor (CMOS) technology-compatible fabrication processes, opens new design spaces towards increased tunability and simplification of the device selection challenge.",2202.04477v2 2019-04-07,Phase field modelling of crack propagation in functionally graded materials,"We present a phase field formulation for fracture in functionally graded materials (FGMs). The model builds upon homogenization theory and accounts for the spatial variation of elastic and fracture properties. Several paradigmatic case studies are addressed to demonstrate the potential of the proposed modelling framework. Specifically, we (i) gain insight into the crack growth resistance of FGMs by conducting numerical experiments over a wide range of material gradation profiles and orientations, (ii) accurately reproduce the crack trajectories observed in graded photodegradable copolymers and glass-filled epoxy FGMs, (iii) benchmark our predictions with results from alternative numerical methodologies, and (iv) model complex crack paths and failure in three dimensional functionally graded solids. The suitability of phase field fracture methods in capturing the crack deflections intrinsic to crack tip mode-mixity due to material gradients is demonstrated. Material gradient profiles that prevent unstable fracture and enhance crack growth resistance are identified: this provides the foundation for the design of fracture resistant FGMs. The finite element code developed can be downloaded from www.empaneda.com/codes.",1904.08749v1 2009-05-13,Reliability of resistivity quantification for shallow subsurface water processes,"The reliability of surface-based electrical resistivity tomography (ERT) for quantifying resistivities for shallow subsurface water processes is analysed. A method comprising numerical simulations of water movement in soil and forward-inverse modeling of ERT surveys for two synthetic data sets is presented. Resistivity contrast, e.g. by changing water content, is shown to have large influence on the resistivity quantification. An ensemble and clustering approach is introduced in which ensembles of 50 different inversion models for one data set are created by randomly varying the parameters for a regularisation based inversion routine. The ensemble members are sorted into five clusters of similar models and the mean model for each cluster is computed. Distinguishing persisting features in the mean models from singular artifacts in individual tomograms can improve the interpretation of inversion results. Especially in the presence of large resistivity contrasts in high sensitivity areas, the quantification of resistivities can be unreliable. The ensemble approach shows that this is an inherent problem present for all models inverted with the regularisation based routine. The results also suggest that the combination of hydrological and electrical modeling might lead to better results.",0905.2117v1 2009-06-17,Resistive MHD jet simulations with large resistivity,"Axisymmetric resistive MHD simulations for radially self-similar initial conditions are performed, using the NIRVANA code. The magnetic diffusivity could occur in outflows above an accretion disk, being transferred from the underlying disk into the disk corona by MHD turbulence (anomalous turbulent diffusivity), or as a result of ambipolar diffusion in partially ionized flows. We introduce, in addition to the classical magnetic Reynolds number Rm, which measures the importance of resistive effects in the induction equation, a new number Rb, which measures the importance of the resistive effects in the energy equation. We find two distinct regimes of solutions in our simulations. One is the low-resistivity regime, in which results do not differ much from ideal-MHD solutions. In the high-resistivity regime, results seem to show some periodicity in time-evolution, and depart significantly from the ideal-MHD case. Whether this departure is caused by numerical or physical reasons is of considerable interest for numerical simulations and theory of astrophysical outflows and is currently investigated.",0906.3254v1 2011-12-29,Magnetospheric Accretion and Ejection of Matter in Resistive Magnetohydrodynamic Simulations,"The ejection of matter in the close vicinity of a young stellar object is investigated, treating the accretion disk as a gravitationally bound reservoir of matter. By solving the resistive MHD equations in 2D axisymmetry using our version of the Zeus-3D code with newly implemented resistivity, we study the effect of magnetic diffusivity in the magnetospheric accretion-ejection mechanism. Physical resistivity was included in the whole computational domain so that reconnection is enabled by the physical as well as the numerical resistivity. We show, for the first time, that quasi-stationary fast ejecta of matter, which we call {\em micro-ejections}, of small mass and angular momentum fluxes, can be launched from a purely resistive magnetosphere. They are produced by a combination of pressure gradient and magnetic forces, in presence of ongoing magnetic reconnection along the boundary layer between the star and the disk, where a current sheet is formed. Mass flux of micro-ejection increases with increasing magnetic field strength and stellar rotation rate, and is not dependent on the disk to corona density ratio and amount of resistivity.",1112.6226v2 2016-10-17,Nonlinear Resistivity for Magnetohydrodynamical Models,"A new formulation of the plasma resistivity that arises from the collisional momentum-transfer rate between electrons and ions is presented. The resistivity computed herein is shown to depend not only on the temperature and density but also on all other polynomial velocity-space moments of the distribution function, such as the pressure tensor and heat flux vector. The exact expression for the collisional momentum-transfer rate is determined, and is used to formulate the nonlinear anisotropic resistivity. The new formalism recovers the Spitzer resistivity, as well as the concept of thermal force if the heat flux is assumed to be proportional to a temperature gradient. Furthermore, if the pressure tensor is related to viscous stress, the latter enters the expression for the resistivity. The relative importance of the nonlinear term(s) with respect to the well-established electron inertia and Hall terms is also examined. The subtle implications of the nonlinear resistivity, and its dependence on the fluid variables, are discussed in the context of magnetized plasma environments and phenomena such as magnetic reconnection.",1610.05193v2 2020-03-09,Quantum mechanical current-to-voltage conversion with quantum Hall resistance array,"Accurate measurement of the electric current requires a stable and calculable resistor for an ideal current to voltage conversion. However, the temporal resistance drift of a physical resistor is unavoidable, unlike the quantum Hall resistance directly linked to the Planck constant h and the elementary charge e. Lack of an invariant high resistance leads to a challenge in making small current measurements below 1 muA with an uncertainty better than one part in 106. In this work, we demonstrate a current to voltage conversion in the range from a few nano amps to one microamp with an invariant quantized Hall array resistance. The converted voltage is directly compared with the Josephson voltage reference in the framework of Ohm's law. Markedly distinct from the classical conversion, which relies on an artifact resistance reference, this current-to-voltage conversion does not demand timely resistance calibrations. It improves the precision of current measurement down to 8 10 -8 at 1 muA.",2003.04464v1 2021-02-11,Suppressing evolution through environmental switching,"Ecology and evolution under changing environments are important in many subfields of biology with implications for medicine. Here, we explore an example: the consequences of fluctuating environments on the emergence of antibiotic resistance, which is an immense and growing problem. Typically, high doses of antibiotics are employed to eliminate the infection quickly and minimize the time under which resistance may emerge. However, this strategy may not be optimal. Since competition can reduce fitness and resistance typically has a reproductive cost, resistant mutants' fitness can depend on their environment. Here we show conditions under which environmental varying fitness can be exploited to prevent the emergence of resistance. We develop a stochastic Lotka-Volterra model of a microbial system with competing phenotypes: a wild strain susceptible to the antibiotic, and a mutant strain that is resistant. We investigate the impact of various pulsed applications of antibiotics on population suppression. Leveraging competition, we show how a strategy of environmental switching can suppress the infection while avoiding resistant mutants. We discuss limitations of the procedure depending on the microbe and pharmacodynamics and methods to ameliorate them.",2102.05813v2 2023-12-08,Electron-hole collision-limited resistance of gapped graphene,"Collisions between electrons and holes can dominate the carrier scattering in clean graphene samples in the vicinity of charge neutrality point. While electron-hole limited resistance in pristine gapless graphene is well-studied, its evolution with induction of band gap $E_g$ is less explored. Here, we derive the functional dependence of electron-hole limited resistance of gapped graphene $\rho_{eh}$ on the ratio of gap and thermal energy $E_g/kT$. At low temperatures and large band gaps, the resistance grows linearly with $E_g/kT$, and possesses a minimum at $E_g \approx 2.5 kT$. This contrast to the Arrhenius activation-type behaviour for intrinsic semiconductors. Introduction of impurities restores the Arrhenius law for resistivity at low temperatures and/or high doping densities. The hallmark of electron-hole collision effects in graphene resistivity at charge neutrality is the crossover between exponential and power-law resistivity scalings with temperature.",2312.05066v1 2019-03-18,"Experimental and Theoretical Investigation on the Possible Half-metallic Behaviour of Equiatomic Quaternary Heusler Alloys: CoRuMnGe and CoRuVZ (Z = Al, Ga)","In this report, structural, electronic, magnetic and transport properties of quaternary Heusler alloys CoRuMnGe and CoRuVZ (Z = Al, Ga) are investigated. All the three alloys are found to crystallize in cubic structure. CoRuMnGe exhibits L2$_1$ structure whereas, the other two alloys have B2-type disorder. For CoRuMnGe and CoRuVGa, the experimental magnetic moments are in close agreement with the theory as well as those predicted by the Slater-Pauling rule, while for CoRuVAl, a relatively large deviation is seen. The reduction in the moment in case of CoRuVAl possibly arises due to the anti-site disorder between Co and Ru sites as well as V and Al sites. Among these alloys, CoRuMnGe has the highest T$\mathrm{_C}$ of 560 K. Resistivity variation with temperature reflects the half-metallic nature in CoRuMnGe alloy. CoRuVAl shows metallic character in both paramagnetic and ferromagnetic states, whereas the temperature dependence of resistivity for CoRuVGa is quite unusual. In the last system, $\rho$ vs. T curve shows an anomaly in the form of a maximum and a region of negative temperature coefficient of resistivity (TCR) in the magnetically ordered state. The ab initio calculations predict nearly half-metallic ferromagnetic state with high spin polarization of 91, 89 and 93 \% for CoRuMnGe, CoRuVAl and CoRuVGa respectively. To investigate the electronic properties of the experimentally observed structure, the Co-Ru swap disordered structures of CoRuMnGe alloy are also simulated and it is found that the disordered structures retain half-metallic nature, high spin polarization with almost same magnetic moment as in the ideal structure. Nearly half-metallic character, high T$\mathrm{_C}$ and high spin polarization make CoRuMnGe alloy promising for room temperature spintronic applications.",1903.07265v2 2021-05-06,High-sensitivity of initial SrO growth on the residual resistivity in epitaxial thin films of SrRuO$_3$ on SrTiO$_3$ (001),"The growth of SrRuO$_3$ (SRO) thin film with high-crystallinity and low residual resistivity (RR) is essential to explore its intrinsic properties. Here, utilizing the adsorption-controlled growth technique, the growth condition of initial SrO layer on TiO$_2$-terminated SrTiO$_3$ (STO) (001) substrate was found to be crucial for achieving a low RR in the resulting SRO film grown afterward. The optimized initial SrO layer shows a $c$(2 x 2) superstructure that was characterized by electron diffraction, and a series of SRO films with different thicknesses ($t$s) were then grown. The resulting SRO films exhibit excellent crystallinity with orthorhombic-phase down to $t \approx$ 4.3 nm, which was confirmed by high resolution X-ray measurements. From azimuthal X-ray scan for SRO orthorhombic (021) reflection, we uncover four structural domains with a dominant domain of orthorhombic SRO [001] along cubic STO [010] direction. The dominant domain population depends on $t$, STO miscut angle (${\alpha}$), and miscut direction (${\beta}$), giving a volume fraction of about 92 $\%$ for $t \approx$ 26.6 nm and (${\alpha}$, ${\beta}$) ~ (0.14$^{\rm o}$, 5$^{\rm o}$). On the other hand, metallic and ferromagnetic properties were well preserved down to $t \approx$ 1.2 nm. Residual resistivity ratio (RRR = ${\rho}$(300 K)/${\rho}$(5 K)) reduces from 77.1 for $t \approx$ 28.5 nm to 2.5 for $t \approx$ 1.2 nm, while ${\rho}$(5 K) increases from 2.5 $\mu\Omega$cm for $t \approx$ 28.5 nm to 131.0 $\mu\Omega$cm for $t \approx$ 1.2 nm. The ferromagnetic onset temperature ($T_c\prime$) of around 151 K remains nearly unchanged down to $t \approx$ 9.0 nm and decreases to 90 K for $t \approx$ 1.2 nm. Our finding thus provides a practical guideline to achieve high crystallinity and low RR in ultra-thin SRO films by simply adjusting the growth of initial SrO layer.",2105.02404v1 2021-12-01,"Synthesis and study of (Na, Zr) and (Ca, Zr) phosphate-molybdates and phosphate-tungstates: Thermal expansion behavior, radiation test and hydrolytic stability","Thermal expansion behavior at high temperatures of synthesized Na$_{1-x}$Zr$_2$(PO$_4$)$_{3-x}$(XO$_4$)$_x$, and Ca$_{1-x}$Zr$_2$(PO$_4$)$_{3-x}$(XO$_4$)$_x$, X = Mo, W compounds has been investigated. Ceramics with relatively high density (more than 97.5%) were produced by Spark Plasma Sintering (SPS) of submicron powders obtained by sol-gel synthesis. The study of strength characteristics has revealed that hardness the ceramics are greater than 5 GPa, and minimum fracture toughness factor was 1 MPa*m$^{1/2}$. It was found that ceramics have a high hydrolytic resistance in the static regime -- the minimum leaching rates for the Mo- and W-containing specimens were $31\times10^{-6}$ and $3.36\times 10^{-6}$ g/(cm$^2$*day), respectively. The ceramics had a high resistance to the irradiation by Xe$^{+26}$ multiple-charged ions with the energy 167 MeV up to the fluences in the range 1*10$^{12}$ - 6*10$^{13}$ cm$^{-2}$. The Mo-containing Na$_{0.5}$Zr$_2$(PO$_4$)$_{2.5}$(XO$_4$)$_{0.5}$ ceramics were shown to have a higher radiation resistance that the phosphate-tungstates.",2112.00373v1 2021-02-22,High T$_C$ ferromagnetic inverse Heusler alloys: A comparative study of Fe$_2$RhSi and Fe$_2$RhGe,"We report the results of experimental investigations on structural, magnetic, resistivity, caloric properties of Fe$_2$RhZ (Z=Si,Ge) along with \textit{ab-initio} band structure calculations using first principle simulations. Both these alloys are found to crystallize in inverse Heusler structure but with disorder in tetrahedral sites between Fe and Rh. Fe$_2$RhSi has saturation moment of 5.00 $\mu_B$ and while its counterpart has 5.19 $\mu_B$. Resistivity measurement reveals metallic nature in both of them. Theoretical simulations using generalized gradient approximation(GGA) predict inverse Heusler structure with ferromagnetic ordering as ground state for both the alloys. However it underestimates the experimentally observed moments. GGA+$U$ approach, with Hubbard $U$ values estimated from density functional perturbation theory helps to improve the comparison of the experimental results. Fe$_2$RhSi is found to be half metallic ferromagnet while Fe$_2$RhGe is not. Varying $U$ values on Fe and Rh sites does not change the net moment much in Fe$_2$RhSi, unlike in Fe$_2$RhGe. Relatively small exchange splitting of orbitals in Fe$_2$RhGe compared to that of Fe$_2$RhSi is the reason for not opening the band gap in the minority spin channel in the former. High ordering temperature and moment make Fe$_2$RhSi useful for spintronics applications.",2102.10967v1 1995-11-10,Contrasting Dynamic Spin Susceptibility Models and their Relation to High Temperature Superconductivity,"We compare the normal-state resistivities $\rho$ and the critical temperatures $T_c$ for superconducting $d_{x^2-y^2}$ pairing due to antiferromagnetic (AF) spin fluctuation exchange in the context of the two phenomenological dynamical spin susceptibility models, recently proposed by Millis, Monien, and Pines (MMP) and Monthoux and Pines (MP) and, respectively, by Radtke, Ullah, Levin, and Norman (RULN), for the cuprate high-$T_c$ materials. Assuming comparable electronic bandwidths and resistiviies in both models, we show that the RULN model gives a much lower d-wave $T_c$ ($\lsim20$K) than the MMP model (with $T_c\sim100$K). We demonstrate that these profound differences in the $T_c$'s arise from fundamental differences in the spectral weight distributions of the two model susceptibilities and are {\it{not}} primarily caused by differences in the calculational techniques employed by MP and RULN. The MMP model, claimed to fit NMR data in YBCO, exhibits substantial amounts of spin fluctuation spectral weight up to an imposed cut-off of 400meV, whereas, in the RULN model, claimed to fit YBCO neutron scattering data, the weight is narrowly peaked and effectively cut-off by 100meV. Further neutron scattering experiments, to explore the spectral weight distribution at all wavevectors over a sufficiently large excitation energy range, will thus be of crucial importance to resolve the question whether AF spin fluctuation exchange provides a viable mechanism to account for high-$T_c$ superconductivity. The large high-frequency boson spectral weight, needed to generate both a high d-wave $T_c$ and a low normal-state resistivity, also implies large values, of order unity, for the Migdal smallness parameter, thus casting serious doubt on the validity of the very",9511051v1 2011-11-14,High Field (14Tesla) Magneto Transport of Sm/PrFeAsO,"We report high field magneto transport of Sm/PrFeAsO. Below spin density wave transition (TSDW), the magneto-resistance (MR) of Sm/PrFeAsO is positive and increasing with decreasing temperature. The MR of SmFeAsO, is found 16%, whereas the same is 21.5% in case of PrFeAsO, at 2.5 K under applied magnetic field of 14 Tesla (T). In case of SmFeAsO, the variation of isothermal MR with field below 20 K is nonlinear at lower magnetic fields (< 2 Tesla) and the same is linear at moderately higher magnetic fields (H \geq 3.5 T). On the other hand PrFeAsO shows almost linear MR at all temperatures below 20 K. The anomalous behavior of MR being exhibited in PrFeAsO is originated from Dirac cone states. The stronger interplay of Fe and Pr ordered moments is responsible for this distinct behavior. PrFeAsO also shows a hump in resistivity (R-T) with possible conduction band (FeAs) mediated ordering of Pr moments at around 12 K. However the same is absent in SmFeAsO even down to 2 K. Our results of high field magneto-transport of up to 14 Tesla brings about clear distinction between ground states of SmFeAsO and PrFeAsO.",1111.3143v2 2013-02-25,On the specifics of the electrical conductivity anomalies in PVC nanocomposites,"A qualitative model describing the ""anomalous"" features of the conductivity of polymer nanocomposites, in particular, switching to the conducting state in relatively thick (tens of microns or more) of flexible PVC films is considered. In previously published experimental results, change of conductivity by 10 or more orders of magnitude occurred both in the absence of external influences (spontaneously), and under the influence of an applied electric field, as well as other initiating factors (such as uniaxial pressure) . In a model of hopping conduction mechanism it is shown, that switching in the conduction states under the action of external field significantly (by orders of magnitude) below threshold can be associated with a high-resistance state instability that results from the sequence of ""shorting"" (reversible soft breakdown) of narrow insulating gaps between regions with relatively high conductivity. Increasing the field strength in the remaining insulating gaps ultimately leads to the formation of a conducting channel between the external electrodes and switching conductivity of the composite film sample in a state of high conductivity. This cascade model is essentially based on the transition from the usual description of the charge tunneling through single independent insulating gap to take into account correlations between adjacent gaps. In the frame of developed model other ""anomalies"" such as exponential dependence of the resistance on the sample thickness, pressure, and other influences can be qualitative explained. An analogy of the model with a cascading breakdown of avalanche transistors is also considered.",1302.5993v1 2016-12-15,The properties of ultrapure delafossite metals,"Although they were first synthesized in chemistry laboratories nearly fifty years ago, the physical properties of the metals PdCoO2, PtCoO2 and PdCrO2 have only more recently been studied in detail. The delafossite structure contains triangular co-ordinated atomic layers, and electrical transport in the delafossite metals is strongly two-dimensional. Their most notable feature is their in-plane conductivity, which is amazingly high for oxide metals. At room temperature, the conductivity of non-magnetic PdCoO2 and PtCoO2 is higher per carrier than those of any alkali metal and even the most conductive elements, copper and silver. At low temperatures the best crystals have resistivities of a few n{\Omega}cm, corresponding to mean free paths of tens of microns. PdCrO2 is a frustrated antiferromagnetic metal, with magnetic scattering contributing to the resistivity at high temperatures and small gaps opening in the Fermi surface below the N\'eel temperature. There is good evidence that electronic correlations are weak in the Pd/Pt layers but strong in the Co/Cr layers; indeed the Cr layer in PdCrO2 is thought to be a Mott insulator. The delafossite metals therefore act like natural heterostructures between strongly correlated and nearly free electron sub-systems. Combined with the extremely high conductivity, they provide many opportunities to study electrical transport and other physical properties in new regimes. The purpose of this review is to describe current knowledge of these fascinating materials and set the scene for what is likely to be a considerable amount of future research.",1612.04948v1 2017-10-05,Dual-wavelength Photo-Hall effect spectroscopy of deep levels in high resistive CdZnTe with negative differential photoconductivity,"Photo-Hall effect spectroscopy was used in the study of deep levels in high resistive CdZnTe. The monochromator excitation in the photon energy range 0.65-1.77 eV was complemented by a laser diode high-intensity excitation at selected photon energies. A single sample characterized by multiple unusual features like negative differential photoconductivity and anomalous depression of electron mobility was chosen for the detailed study involving measurements at both the steady and dynamic regimes. We revealed that the Hall mobility and photoconductivity can be both enhanced and suppressed by an additional illumination at certain photon energies. The anomalous mobility decrease was explained by an excitation of the inhomogeneously distributed deep level at the energy Ev+1.0 eV enhancing thus potential non-uniformities. The appearance of negative differential photoconductivity was interpreted by an intensified electron occupancy of that level by a direct valence band-to-level excitation. Modified Shockley-Read-Hall theory was used for fitting experimental results by a model comprising five deep levels. Properties of the deep levels and their impact on the device performance were deduced.",1710.01945v1 2020-02-25,"Hydrogenated amorphous silicon detectors for particle detection, beam flux monitoring and dosimetry in high-dose radiation environment","Hydrogenated amorphous silicon (a-Si:H) has remarkable radiation resistance properties and can be deposited on a lot of different substrates. A-Si:H based particle detectors have been built since mid 1980s as planar p-i-n or Schottky diode structures; the thickness of these detectors ranged from 1 to 50 micron. However MIP detection using planar structures has always been problematic due to the poor S/N ratio related to the high leakage current at high depletion voltage and the low charge collection efficiency. The usage of 3D detector architecture can be beneficial for the possibility to reduce inter-electrode distance and increase the thickness of the detector for larger charge generation compared to planar structures. Such a detector can be used for future hadron colliders for its radiation resistance and also for X-ray imaging. Furthermore the possibility of a-Si:H deposition on flexible materials (like kapton) can be exploited to build flexible and thin beam flux measurement detectors and x-ray dosimeters.",2002.10848v1 2021-01-29,Wide-range epitaxial strain control of electrical and magnetic properties in high-quality SrRuO3 films,"Epitaxial strain in 4d ferromagnet SrRuO3 films is directly linked to the physical properties through the strong coupling between lattices, electrons, and spins. It provides an excellent opportunity to tune the functionalities of SrRuO3 in electronic and spintronic devices. However, a thorough understanding of the epitaxial strain effect in SrRuO3 has remained elusive due to the lack of systematic studies. This study demonstrates wide-range epitaxial strain control of electrical and magnetic properties in high-quality SrRuO3 films. The epitaxial strain was imposed by cubic or pseudocubic perovskite substrates having a lattice mismatch of -1.6 to 2.3% with reference to bulk SrRuO3. The Poisson ratio, which describes the two orthogonal distortions due to the substrate clamping effect, is estimated to be 0.33. The Curie temperature (TC) and residual resistivity ratios of the series of films are higher than or comparable to the highest reported values for SrRuO3 on each substrate, confirming the high crystalline quality of the films. A TC of 169 K is achieved in a tensile-strained SrRuO3 film on the DyScO3 (110) substrate, which is the highest value ever reported for SrRuO3. The TC (146-169 K), magnetic anisotropy (perpendicular or in-plane magnetic easy axis), and metallic conduction (residual resistivity at 2 K of 2.10 - 373 {\mu}{\Omega}cm) of SrRuO3 are widely controlled by epitaxial strain. These results provide guidelines to design SrRuO3-based heterostructures for device applications.",2101.12376v1 2020-05-16,Pressure-induced Topological and Structural Phase Transitions in an Antiferromagnetic Topological Insulator,"Recently, natural van der Waals heterostructures of (MnBi2Te4)m(Bi2Te3)n have been theoretically predicted and experimentally shown to host tunable magnetic properties and topologically nontrivial surface states. In this work, we systematically investigate both the structural and electronic responses of MnBi2Te4 and MnBi4Te7 to external pressure. In addition to the suppression of antiferromagnetic order, MnBi2Te4 is found to undergo a metal-semiconductor-metal transition upon compression. The resistivity of MnBi4Te7 changes dramatically under high pressure and a non-monotonic evolution of \r{ho}(T) is observed. The nontrivial topology is proved to persists before the structural phase transition observed in the high-pressure regime. We find that the bulk and surface states respond differently to pressure, which is consistent with the non-monotonic change of the resistivity. Interestingly, a pressure-induced amorphous state is observed in MnBi2Te4, while two high pressure phase transitions are revealed in MnBi4Te7. Our combined theoretical and experimental research establishes MnBi2Te4 and MnBi4Te7 as highly tunable magnetic topological insulators, in which phase transitions and new ground states emerge upon compression.",2005.08015v1 2020-08-03,Solute hydrogen and deuterium observed at the near atomic scale in high-strength steel,"Observing solute hydrogen (H) in matter is a formidable challenge, yet, enabling quantitative imaging of H at the atomic-scale is critical to understand its deleterious influence on the mechanical strength of many metallic alloys that has resulted in many catastrophic failures of engineering parts and structures. Here, we report on the APT analysis of hydrogen (H) and deuterium (D) within the nanostructure of an ultra-high strength steel with high resistance to hydrogen embrittlement. Cold drawn, severely deformed pearlitic steel wires (Fe-0.98C-0.31Mn-0.20Si-0.20Cr-0.01Cu-0.006P-0.007S wt.%, {\epsilon}=3.1) contains cementite decomposed during the pre-deformation of the alloy and ferrite. We find H and D within the decomposed cementite, and at some interfaces with the surrounding ferrite. To ascertain the origin of the H/D signal obtained in APT, we explored a series of experimental workflows including cryogenic specimen preparation and cryogenic-vacuum transfer from the preparation into a state-of-the-art atom probe. Our study points to the critical role of the preparation, i.e. the possible saturation of H-trapping sites during electrochemical polishing, how these can be alleviated by the use of an outgassing treatment, cryogenic preparation and transfer prior to charging. Accommodation of large amounts of H in the under-stoichiometric carbide likely explains the resistance of pearlite against hydrogen embrittlement.",2008.00684v1 2021-07-01,"Singular angular magnetoresistance and sharp resonant features in a high-mobility metal with open orbits, ReO3","We report high-resolution angular magnetoresistance (AMR) experiments performed on crystals of ReO$_3$ with high mobility (90,000 cm$^2$/Vs at 2 K) and extremely low residual resistivity (5-8 n$\Omega$cm). The Fermi surface, comprised of intersecting cylinders, supports open orbits. The resistivity $\rho_{xx}$ in a magnetic field $B$ = 9 T displays a singular pattern of behavior. With $\bf E\parallel \hat{x}$ and $\bf B$ initially $\parallel\bf\hat{z}$, tilting $\bf B$ in the longitudinal $k_z$-$k_x$ plane leads to a steep decrease in $\rho_{xx}$ by a factor of 40. However, if $\bf B$ is tilted in the transverse $k_y$-$k_z$ plane, $\rho_{xx}$ increases steeply by a factor of 8. Using the Shockley tube integral approach, we show that, in ReO$_3$, the singular behavior results from the rapid conversion of closed to open orbits, resulting in opposite signs for AMR in orthogonal planes. The floor values of $\rho_{xx}$ in both AMR scans are identified with specific sets of open and closed orbits. Also, the ""completion angle"" $\gamma_c$ detected in the AMR is shown to be an intrinsic geometric feature that provides a new way to measure the Fermi radius $k_F$. However, additional sharp resonant features which appear at very small tilt angles in the longitudinal AMR scans are not explained by the tube integral approach.",2107.00742v1 2021-07-07,Development and validation of electrical-insulating Al2O3 coatings for high-temperature liquid PbLi applications,"Electrical-insulating coatings are of great importance for liquid-metal breeder/coolant based systems relevant to fusion power plants. In specific to Pb-16Li eutectic, a candidate breeder material, such coatings are being actively investigated for their criticality in addressing various functionalities. For such applications, a candidate coating must be demonstrated for its compatibility with corrosive media, high operational temperatures and integrity of electrical-insulation over long durations without substantial degradation. At present, no relevant in-situ insulation resistance (IR) data is available for performance assessment of coated substrates within PbLi environment. To address this shortfall, an experimental study was performed at IPR towards application of high-purity alumina coatings on SS-316L substrates and further rigorous validation in static PbLi environment. The adopted coating process required a low-temperature heat treatment (< 430C) and could yield average coating thicknesses in the range of 100-500 micron. Coated samples were validated for their electrical insulation integrity in static PbLi over two test campaigns for continuous durations of over 700 h and 1360 h, including thermal cycling, at operational temperature between 300C-400C. Estimated volumetric electrical-resistivity remained of the order of 109-1011 ohm-cm without significant degradation. In-situ estimations of thermal derating factors establish excellent electrical-insulation characteristics after long term exposure to liquid PbLi. This paper presents details of utilized coating application methods, coating thickness estimations, liquid-metal test set-up, insulation performance and critical observations from SEM/EDX and XRD analysis on the tested samples.",2107.03244v1 2021-09-26,Tomographic Volumetric Additive Manufacturing of Silicon Oxycarbide Ceramics,"Ceramics are highly technical materials with properties of interest for multiple industries. Precisely because of their high chemical, thermal, and mechanical resistance, ceramics are difficult to mold into complex shapes. A possibility to make convoluted ceramic parts is to use preceramic polymers (PCP) in liquid form. The PCP resin is first solidified in a desired geometry and then transformed into ceramic compounds through a pyrolysis step that preserves the shape. Light-based additive manufacturing (AM) is a promising route to achieve solidification of the PCP resin. Different approaches, such as stereolithography, have already been proposed but they all rely on a layer-by-layer printing process which sets limitations on the printing speed and object geometry. Here, we report on the fabrication of complex 3D centimeter-scale ceramic parts by using tomographic volumetric printing which is fast, high resolution and offers a lot of freedom in terms of geometrical design compared to state-of-the-art AM techniques. First, we formulated a photosensitive preceramic resin that was solidified by projecting light patterns from multiple angles. Then, the obtained 3D printed parts were converted into ceramics by pyrolyzing them in a furnace. We demonstrate the strength of this approach through the fabrication of dense microcomponents exhibiting overhangs and hollow geometries without the need of supporting structures, and characterize their resistance to high heat and harsh chemical treatments.",2109.12680v1 2022-11-16,Characterisation of Gamma-irradiated MCz-Silicon Detectors with a High-$K$ Negative Oxide as Field Insulator,"The high-luminosity operation of the Tracker in the Compact Muon Solenid (CMS) detector at the Large Hadron Collider (LHC) experiment calls for the development of silicon-based sensors. This involves implementation of AC-coupling to micro-scale pixel sensor areas to provide enhanced isolation of radiation-induced leakage currents. The motivation of this study is the development of AC-pixel sensors with negative oxides (such as aluminium oxide - Al$_2$O$_3$ and hafnium oxide - HfO$_2$) as field insulators that possess good dielectric strength and provide radiation hardness. Thin films of Al$_2$O$_3$ and HfO$_2$ grown by atomic layer deposition (ALD) method were used as dielectrics for capacitive coupling. A comparison study based on dielectric material used in MOS capacitors indicate HfO$_2$ as a better candidate since it provides higher sensitivity (where, the term sensitivity is defined as the ratio of the change in flat-band voltage to dose) to negative charge accumulation with gamma irradiation. Further, space charge sign inversion was observed for sensors processed on high resistivity p-type Magnetic Czochralski silicon (MCz-Si) substrates that were irradiated with gamma rays up to a dose of 1 MGy. The inter-pixel resistance values of heavily gamma irradiated AC-coupled pixel sensors suggest that high-$K$ negative oxides as field insulators provide a good electrical isolation between the pixels.",2211.09158v2 2023-07-12,Extrinsic Anomalous Hall effect in Mn Doped GeSnTe Semiconductors in the Bad Metal Hopping Regime,"We present high field magnetotransport studies of Ge1-x-y(SnxMny)Te bulk multiferroics with diamagnetic Sn and paramagnetic Mn concentration x = 0.38 to 0.79 and y = 0.02 to 0.086, respectively. The zero field resistivity, {\rho}(T) takes significant contribution from defects below T = 20 K however, a mixed scattering contribution from dynamic disorder and unusual sources is estimated from T = 20 K to 300 K. The carrier mobility shows anomalous temperature dependence from T0.2 to T0.5 which hints towards possible presence of polaronic effects resulting from coupling of holes with phonons. This anomalous behavior cannot be understood in terms of pure phononic scattering mechanism at high temperature. From point of view of high field results, the transverse component of magnetoresistivity manifests anomalous Hall effect originating from extrinsic scattering sources, particularly the side jump mechanism reveals a larger contribution. We also find that the correlation between the transverse and longitudinal conductivities follow the universal scaling law {\sigma}xy ~ {\sigma}xxn where n = 1.6 in the low conductivity limit. The values n = 1.5 to 1.8 obtained for the present GSMT alloys justify the bad metal hopping regime since the results fall in the low conductivity ferromagnetic family with {\sigma}xx ~ 104 ohmcm-1. The interpretation of the n = 1.6 scaling in the low conductivity regime is thus far not fully understood. However, the anomalous Hall resistivity scaling with modified relation by Tian et al is indicative of the dominant side jump scattering along with noticeable role of skew scattering.",2307.06271v1 2012-10-07,Tailoring Magnetism of Perpendicularly Magnetized MnxGa Epitaxial Films on GaAs for Practical Applications,"MnxGa films with high perpendicular anisotropy, coercivity and energy product have great application potential in ultrahigh-density perpendicular recording, permanent magnets, spin-transfer-torque memory and oscillators, magneto-resistance sensors and ferromagnetic metal/semiconductor heterostructure devices. Here we present a comprehensive diagram of effective magnetism-tailoring of perpendicularly magnetized MnxGa films grown on III-V semiconductor GaAs by using molecular-beam epitaxy for the first time, by systematically investigating the wide-range composition and detailed post-growth annealing effects. We show that the (001)-orientated MnxGa films with L10 or D022 ordering could be crystallized on GaAs in a very wide composition range from x=0.76 to 2.6. L10-ordered MnxGa films show robust magnetization, high remanent ratio, giant perpendicular anisotropy, high intrinsic and extrinsic coercivity, and large energy product, which make this kind of material favorable for perpendicular magnetic recording, high-performance spintronic devices and permanent magnet applications. In contrast, D022-ordered films exhibit lower perpendicular anisotropy and weaker magnetism. Post-growth annealing MnxGa films studies reveal high thermal-stability up to 450 oC, and effective tailoring of magnetic properties can be realized by prolonging annealing at 450 oC. These results would be helpful for understanding this kind of material and designing new spintronic devices for specific practical applications.",1210.2062v3 2012-11-14,The Critical Current Density of an SNS Josephson-Junction,"The critical current density (Jc) through a superconductor in high magnetic fields is controlled by the inclusions and microstructure of the material that hold fluxons stationary to keep the resistance zero and is described using Ginzburg-Landau (G-L) theory. Although the functional form of Jc for superconducting-normal-superconducting (SNS) Josephson-Junctions (J-Js) is known in the low field limit, includes the local properties of the junctions and has been confirmed experimentally in many systems, there are no general solutions for Jc of J-Js in high fields. Scaling laws describe the functional form (magnetic field, temperature and strain dependence) of Jc for polycrystalline superconductors in high fields but do not include local grain boundary properties. They are derived by considering isolated pinning sites where at criticality fluxons either depin or free fluxons shear past pinned fluxons as part of the flux line lattice. However, visualisation of solutions to the Time Dependent Ginzburg-Landau (TDGL) equations for polycrystalline materials have shown that fluxons cross the superconductor by flowing along the grain boundaries. Here we derive clean- and dirty- limit analytic equations for of SNS J-Js in high fields and verify them using computational solutions to TDGL theory. We consider SNS J-Js to be the basic building blocks for grain boundaries in polycrystalline materials since they provide flux-flow channels. The J-Js description provides a mathematical framework that includes the utility of scaling laws together with our microscopic understanding of barriers to supercurrent flow and helps identify the grain boundary engineering that can improve in low temperature polycrystalline superconductors used in high magnetic field applications.",1211.3255v2 2013-09-08,Nanoscale resolution scanning thermal microscopy with thermally conductive nanowire probes,"Scanning thermal microscopy (SThM) - a type of scanning probe microscopy that allows mapping thermal transport and temperatures in nanoscale devices, is becoming a key approach that may help to resolve heat dissipation problems in modern processors and develop new thermoelectric materials. Unfortunately, performance of current SThM implementations in measurement of high thermal conductivity materials continues to me limited. The reason for these limitations is two-fold - first, SThM measurements of high thermal conductivity materials need adequate high thermal conductivity of the probe apex, and secondly, the quality of thermal contact between the probe and the sample becomes strongly affected by the nanoscale surface corrugations of the studied sample. In this paper we develop analytical models of the SThM approach that can tackle these complex problems - by exploring high thermal conductivity nanowires as a tip apex, and exploring contact resistance between the SThM probe and studied surface, the latter becoming particularly important when both tip and surface have high thermal conductivities. We develop analytical model supported by the finite element analysis simulations and by the experimental tests of SThM prototype using carbon nanotube (CNT) at the tip apex as a heat conducting nanowire. These results elucidate vital relationships between the performance of the probe in SThM from one side and thermal conductivity, geometry of the probe and its components from the other, providing pathway for overcoming current limitations of SThM.",1309.2010v1 2019-09-13,Electric field and current induced electroforming modes in NbOx,"Electroforming is used to initiate the memristive response in metal/oxide/metal devices by creating a filamentary conduction path in the oxide film. Here we use a simple photoresist-based detection technique to map the spatial distribution of conductive filaments formed in Nb/NbOx/Pt devices, and correlate these with current-voltage characteristics and in-situ thermoreflectance measurements to identify distinct modes of electroforming in low and high conductivity NbOx films. In low conductivity films the filaments are randomly distributed within the oxide film, consistent with a field-induced weakest-link mechanism, while in high conductivity films they are concentrated in the center of the film. In the latter case the current-voltage characteristics and in-situ thermoreflectance imaging show that electroforming is associated with current bifurcation into regions of low and high current density. This is supported by finite element modelling of the current distribution and shown to be consistent with predictions of a simple core-shell model of the current distribution. These results clearly demonstrate two distinct modes of electroforming in the same materials system and show that the dominant mode depends on the conductivity of the film, with field-induced electroforming dominant in low conductivity films and current-bifurcation induced electroforming dominant in high conductivity films. Finally, we demonstrate S-type and snap-back negative differential resistance in the high conductivity films and explain this behavior in terms of two-zone model.",1909.06443v2 2000-05-25,Critical Resistivity along the Quantum Hall Liquid--Insulator Transition Line,"The critical resistivity measured along the quantum Hall liquid--insulator transition line indicates a pronounced peak at a critical filling factor close to 1, which marks the crossover from the high to low magnetic field regime in the phase diagram. The origin of this behavior is explained in the framework of classical transport in a puddle network model. The proposed scenario is also consistent with the behavior of the critical Hall resistance along the transition line. In addition, a formula is suggested as a fit for isotherms ($\rho_{xx}$ vs. $\nu$) in the moderately high field regime, which exhibits a violation of duality symmetry as the critical resistivity is evelated from the `universal' value $h/e^2$.",0005436v1 2018-03-20,HPL-GEM: Controlling High Pressure Laminates bulk resistivity with GEMs,"We succeeded in modifying and controlling the electrical resistance of a standard High Pressure Laminate (HPL) panel through the use of a Gas Electron Multiplier (GEM) foil that has been embedded into the bulk of the HPL plate itself. Electrical characterizations were made and preliminary data show that this HPL-GEM embedded system can easily vary its bulk resistance by more than one order of magnitude. Data show that the bulk resistance change is exponential with the applied voltage to the embedded GEM.",1803.07675v1 2024-02-22,Auxiliary Calculations for Graphene-Based Quantum Hall Arrays Using Partially Recursive Star-Mesh Transformations,"A previous mathematical approach adopted for optimizing the number of total device elements required for obtaining high effective quantized resistances in graphene-based quantum Hall array devices (QHARS) has been further explored with partial recursion patterns. Designs would assume the use of epitaxial graphene elements, whose quantized Hall resistance at the {\nu}=2 plateau (R_H \approx 12906.4 \Ohm) becomes the building block for larger effective, quantized resistances. Auxiliary calculations suggest the importance of applying full recursions at least once to maximize the reduction of total QHARS elements needed for high resistances.",2402.14520v1 2005-03-31,Tuning Negative Differential Resistance in a Molecular Film,"We have observed tunable negative differential resistance (NDR) in scanning tunneling spectroscopy measurements of a double layer of C60 molecules on a metallic surface. Using a simple model we show that the observed NDR behavior is explained by voltage-dependent changes in the tunneling barrier height.",0503765v1 2006-10-10,Residual resistivity due to wedge disclination dipoles in metals with rotational plasticity,"The residual resistivity $\rho $ in metals caused by wedge disclination dipoles is studied in the framework of the Drude formula. It is shown that $\rho\sim L^{-p}$ with $p=3$ for biaxial and $p=2$ for uniaxial dipoles ($L$ is a size of dipole arm)",0610258v1 2006-10-26,Two years later--lessons from vortex dynamics in super media,"Two years ago the reasons for resistance to the fundamental vortex dynamics in super media emerged in 1990's were analyzed (cond-mat/0407007). Five ""mistakes"" were identified to explain this resistance. Given the current tremendous interest in vortex dynamics, it would be desirable to provide a progress report: A survey of literature reveals that 3 out 5 ""mistakes"" has in fact been confirmed by other researchers.",0610753v1 2008-12-16,Electrical properties of vanadium oxide subject to hydrogen plasma treatment,"The effect of doping with hydrogen on the electrical properties of vanadium oxide is studied. For vanadium oxide films, subject to cold hydrogen plasma treatment, the temperature dependence of resistance with a maximum at T ~ 100 K is observed. Also, the dependence of the a.c. resistance on frequency is studied. A strategy for fabrication new superconducting materials is discussed.",0812.2973v1 2011-02-07,Direct correlation between strengthening mechanisms and electrical noise in strained copper wires,"We have measured the resistance noise of copper metallic wires during a tensile stress. The time variation of the main resistance is continuous up to the wire breakdown, but its fluctuations reveal the intermittent and heterogeneous character of plastic flow. We show in particular direct correlations between strengthening mechanisms and noise spectra characteristics.",1102.1253v1 2011-09-05,Mesoscopic Thermovoltage Measurement Design,"Quantitative thermoelectric measurements in the mesoscopic regime require accurate knowledge of temperature, thermovoltage, and device energy scales. We consider the effect of a finite load resistance on thermovoltage measurements of InAs/InP heterostructure nanowires. Load resistance and ac attenuation distort the measured thermovoltage therefore complicating the evaluation of device performance. Understanding these effects improves experimental design and data interpretation.",1109.1009v1 2016-07-20,MegaOhm Extraordinary Hall effect in oxidized CoFeB,"We report on development of controllably oxidized CoFeB ferromagnetic films demonstrating the extraordinary Hall effect (EHE) resistivity exceeding 1 Ohmcm and magnetic field sensitivity up to 10^6 Ohm/T. Such EHE resistivity is four orders of magnitude higher than previously observed in ferromagnetic materials, while sensitivity is two orders larger than the best of semiconductors",1607.05923v1 1995-12-18,Anisotropic Localization Effect in Layered Materials,"We investigate localization properties in the highly anisotropic and intrinsically disordered layered material, which is analogous to high-Tc cuprates. By varying the anisotropy of the system which is parameterized by the interlayer hopping $tp$, we find a crossover from two-dimensional (2D) to three-dimensional (3D) behavior at a critical hopping amplitude $tp_c$, where a mobility edge starts to appear. We show that below the mobility edge, anisotropic localization effect may exist for a finite size system, when the $ab$-plane localization length is longer than the system size and the $c$-axis localization length is shorter than the system size. Nevertheless, we argue that such anisotropic localization can not account for the ``semiconductor'' like behavior of the $c$-axis resistivity of high $\Tc$ cuprates.",9512133v1 2008-03-20,Graphene-Based Liquid Crystal Device,"Graphene is only one atom thick, optically transparent, chemically inert and an excellent conductor. These properties seem to make this material an excellent candidate for applications in various photonic devices that require conducting but transparent thin films. In this letter we demonstrate liquid crystal devices with electrodes made of graphene which show excellent performance with a high contrast ratio. We also discuss the advantages of graphene compared to conventionally-used metal oxides in terms of low resistivity, high transparency and chemical stability.",0803.3031v1 2008-10-02,Carrier doping to pseudo-low-dimensional compound La2RuO5,"Hole carrier doping has been tried to pseudo-low-dimensional material La2RuO5 by substituting La3+ with Cd2+. Single phased samples of La2-xCdxRuO5 with x up to 0.5 have been successfully obtained and also high pressure O2 annealing has been performed to the x=0.5 sample. Although the formal ionic state of Ru is expected to increase from 4+ (at x=0) to 4.5+ (at x=0.5), the magnetic and electrical properties show no significant changes in as-sintered samples. In contrast, high pressure O2 annealed x=0.5 samples show a little reduction of electrical resistivity and the decrease of thermoelectric power at 260 K. From these results, it can be speculated that the doped carriers are mostly compensated by oxygen deficiency in as-sintered samples.",0810.0350v1 2008-12-15,"High-temperature oxygen non-stoichiometry, conductivity and structure in strontium-rich nickelates La2-xSrxNiO4-δ(x = 1 and 1.4)","Oxygen nonstoichiometry, electrical conductivity and thermal expansion of La2 xSrxNiO4-\delta phases with high levels of strontium substitution (1 =< x =< 1.4) have been investigated in air and oxygen atmosphere in the temperature range 20-1050 degrees C. These phases retain the K2NiF4-type structure of La2NiO4 (tetragonal, space group I4/mmm). The oxygen vacancy fraction was determined independently from thermogravimetric and neutron diffraction experiments, and is found to increase considerably on heating. The electrical resistivity, thermal expansion and cell parameters with temperature show peculiar variations with temperature, and differ notably from La2NiO4$\pm$\delta in this respect. These variations are tentatively correlated with the evolution of nickel oxidation state, which crosses from a Ni3+/Ni4+ to a Ni2+/Ni3+ equilibrium on heating.",0812.2747v1 2009-12-08,The Deposition of High-Quality HfO2 on Graphene and the Effect of Remote Oxide Phonon Scattering,"We demonstrate the atomic layer deposition of high-quality HfO2 film on graphene and report the magnitude of remote oxide phonon (ROP) scattering in dual-oxide graphene transistors. Top gates with 30 nm HfO2 oxide layer exhibit excellent doping capacity of greater than 1.5x10^(13)/cm^(2). The carrier mobility in HfO2-covered graphene reaches 20,000 cm^(2)/Vs at low temperature, which is the highest among oxide-covered graphene and compares to that of pristine samples. The temperature-dependent resistivity exhibits the effect of ROP scattering from both the SiO2 substrate and the HfO2 over-layer. At room temperature, surface phonon modes of the HfO2 film centered at 54 meV dominate and limit the carrier mobility to ~20,000 cm^(2)/Vs. Our results highlight the important choice of oxide in graphene devices.",0912.1378v2 2013-12-21,Near-Field Microwave Magnetic Nanoscopy of Superconducting Radio Frequency Cavity Materials,"A localized measurement of the RF critical field on superconducting radio frequency (SRF) cavity materials is a key step to identify specific defects that produce quenches of SRF cavities. Two new measurements are performed to demonstrate these capabilities with a novel near-field scanning probe microwave microscope. The first is a third harmonic nonlinear measurement on a high Residual- Resistance-Ratio bulk Nb sample showing strong localized nonlinear response for the first time, with surface RF magnetic field $B_{surface} \sim 10^{2}$ $mT$. The second is a raster scanned harmonic response image on a high quality $MgB_{2}$ thin film demonstrating a quench defect-free surface over large areas.",1312.6257v1 2014-11-14,"Characterization of TiAlSiON Coatings Deposited by Plasma Enhanced Magnetron Sputtering: XRD, XPS, and DFT Studies","The results of characterization of TiAlSiON hard coatings deposited on ferric-chromium AISI 430 stainless steel by plasma enhanced magnetron sputtering are presented. The coating with maximum hardness (of 45 GPa) was obtained at the following optimal values of elemental concentrations: Si ~5 at.%, Al ~15 at.%, and Ti ~27 at.%. The elastic modulus of the coating was 590 GPa. The reading of gaseous mixture (Ar-N2) pressure was 1*10-3 Torr and the reading of partial pressure of oxygen (O2) was 1*10-5 Torr. The X-ray diffraction (XRD) measurements showed the presence of Ti(Al)N. High-energy resolved XPS spectra of core levels revealed the formation of Ti-N, Ti-O-N, Si-N and Al-O-N bonds. Comparison of XPS valence band spectra with specially performed density functional theory calculations for two ordered and few disordered TiN1-xOx (0 =< x <= 1) demonstrates that a Ti(Al)OxNy phase is formed on the surface of AISI430 steel upon the plasma enhanced magnetron sputtering, which provides this material with a good combination of high hardness and improved oxidation resistance.",1411.3859v1 2015-05-25,Cluster spin-glass ground state in quasi-one-dimensional KCr$_{3}$As$_{3}$,"We report structural and physical properties of a new quasi-one-dimensional Cr-based compound, KCr$_{3}$As$_{3}$, which is prepared by potassium deintercalation from the superconductive K$_{2}$Cr$_{3}$As$_{3}$. KCr$_{3}$As$_{3}$ adopts the TlFe$_{3}$Te$_{3}$-type structure with space group $P6_{3}$/$m$ (No. 176). The high-temperature magnetic susceptibility obeys the Curie-Weiss law with an effective magnetic moment of 0.68 $\mu_{\mathrm{B}}$/Cr. Below 56 K the susceptibility deviates from the high-temperature Curie-Weiss behavior, coinciding with the rapid increase in resistivity, which suggests formation of spin clusters. The short-range spin correlations are also supported by the specific-heat data. The title material does not exhibit bulk superconductivity; instead, it shows a cluster spin-glass state below $\sim$ 5 K.",1505.06525v1 2017-12-29,Structural transformations in porous glasses under mechanical loading. II. Compression,"The role of porous structure and glass density in response to compressive deformation of amorphous materials is investigated via molecular dynamics simulations. The disordered, porous structures were prepared by quenching a high-temperature binary mixture below the glass transition into the phase coexistence region. With decreasing average glass density, the pore morphology in quiescent samples varies from a random distribution of compact voids to a porous network embedded in a continuous glass phase. We find that during compressive loading at constant volume, the porous structure is linearly transformed in the elastic regime and the elastic modulus follows a power-law increase as a function of the average glass density. Upon further compression, pores deform significantly and coalesce into large voids leading to formation of domains with nearly homogeneous glass phase, which provides an enhanced resistance to deformation at high strain.",1712.10265v1 2018-02-07,"Stability of boron-doped graphene/copper interface: DFT, XPS and OSEE studies","Two different types of boron-doped graphene/copper interfaces synthesized using two different flow rates of Ar through the bubbler containing the boron source were studied. X-ray photoelectron spectra (XPS) and optically stimulated electron emission (OSEE) measurements have demonstrated that boron-doped graphene coating provides a high corrosion resistivity of Cu-substrate with the light traces of the oxidation of carbon cover. The density functional theory calculations suggest that for the case of substitutional (graphitic) boron-defect only the oxidation near boron impurity is energetically favorable and creation of the vacancies that can induce the oxidation of copper substrate is energetically unfavorable. In the case of non-graphitic boron defects oxidation of the area, a nearby impurity is metastable that not only prevent oxidation but makes boron-doped graphene. Modeling of oxygen reduction reaction demonstrates high catalytic performance of these materials.",1802.02345v1 2018-06-11,Uncovering electron scattering mechanisms in NiFeCoCrMn derived concentrated solid solution and high entropy alloys,"Whilst it has long been known that disorder profoundly affects transport properties, recent measurements on a series of solid solution 3d-transition metal alloys reveal two orders of magnitude variations in the residual resistivity. Using ab-initio methods, we demonstrate that, while the carrier density of all alloys is as high as in normal metals, the electron mean-free-path can vary from ~10 {\AA} (strong scattering limit) to ~10$^3$ {\AA} (weak scattering limit). Here, we delineate the underlying electron scattering mechanisms responsible for this disparate behavior. While spin dependent site-diagonal disorder is always dominant, for alloys containing only Fe, Co, and Ni the majority spin channel experiences negligible disorder scattering, thereby providing a short circuit, while for Cr/Mn containing alloys both spin channels experience strong disorder scattering due to an electron filling effect. Unexpectedly, other scattering mechanisms (e.g. displacement scattering) are found to be relatively weak in most cases.",1806.03785v2 2018-11-26,Engineering Large Anisotropic Magnetoresistance in La0.7Sr0.3MnO3 Films at Room Temperature,"The magnetoresistance (MR) effect is widely employed in technologies that pervade our world from magnetic reading heads to sensors. Diverse contributions to MR, such as anisotropic, giant, tunnel, colossal, and spin-Hall, are revealed in materials depending on the specific system and measuring configuration. Half-metallic manganites hold promise for spintronic applications but the complexity of competing interactions has not permitted the understanding and control of their magnetotransport properties to enable the realization of their technological potential. Here we report on the ability to induce a dominant switchable magnetoresistance in La0.7Sr0.3MnO3 epitaxial films, at room temperature (RT). By engineering an extrinsic magnetic anisotropy, we show a large enhancement of anisotropic magnetoresistance (AMR) which leads to, at RT, signal changes much larger than the other contributions such as the colossal magnetoresistance (CMR). The dominant extrinsic AMR exhibits large variation in the resistance in low field region, showing high sensitivity to applied low magnetic fields. These findings have a strong impact on the real applications of manganite based devices for the high-resolution low field magnetic sensors or spintronics.",1811.10301v1 2017-03-23,Unconventional Large Linear Magnetoresistance in Cu$_{2-x}$Te,"We report a large linear magnetoresistance in Cu$_{2-x}$Te, reaching $\Delta\rho/\rho(0)$ = 250\% at 2 K in a 9 T field. This is observed for samples with $x$ in the range 0.13 to 0.22, and the results are comparable to the effects observed in Ag$_2 X$ materials, although in this case the results appear for a much wider range of bulk carrier density. Examining the magnitude vs. crossover field from low-field quadratic to high-field linear behavior, we show that models based on classical transport behavior best explain the observed results. The effects are traced to misdirected currents due to topologically inverted behavior in this system, such that stable surface states provide the high mobility transport channels. The resistivity also crosses over to a $T^2$ dependence in the temperature range where the large linear MR appears, an indicator of electron-electron interaction effects within the surface states. Thus this is an example of a system in which these interactions dominate the low-temperature behavior of the surface states.",1703.07945v1 2019-02-14,One-dimensional edge contacts to a monolayer semiconductor,"Integration of electrical contacts into van der Waals (vdW) heterostructures is critical for realizing electronic and optoelectronic functionalities. However, to date no scalable methodology for gaining electrical access to buried monolayer two-dimensional (2D) semiconductors exists. Here we report viable edge contact formation to hexagonal boron nitride (hBN) encapsulated monolayer MoS$_2$. By combining reactive ion etching, in situ Ar$^+$ sputtering and annealing, we achieve a relatively low edge contact resistance, high mobility (up to ~30 cm$^2$/Vs) and high on-current density (>50 uA/um at V$_{\rm DS}$ = 3V), comparable to top contacts. Furthermore, the atomically smooth hBN environment also preserves the intrinsic MoS$_2$ channel quality during fabrication, leading to a steep subthreshold swing of 116 mV/dec with a negligible hysteresis. Hence, edge contacts are highly promising for large-scale practical implementation of encapsulated heterostructure devices, especially those involving air sensitive materials, and can be arbitrarily narrow, which opens the door to further shrinkage of 2D device footprint.",1902.05506v3 2019-02-20,Vortex pinning and flux flow microwave studies of coated conductors,"Demanding microwave applications in a magnetic field require the material optimization not only in zero-field but, more important, in the in-field flux motion dominated regime. However, the effect of artificial pinning centers (APC) remains unclear at high frequency. Moreover, in coated conductors the evaluation of the high frequency material properties is difficult due to the complicated electromagnetic problem of a thin superconducting film on a buffered metal substrate. In this paper we present an experimental study at 48 GHz of 150-200 nm YBa$_2$Cu$_3$O$_{7-x}$ coated conductors, with and without APCs, on buffered Ni-5at%W tapes. By properly addressing the electromagnetic problem of the extraction of the superconductor parameters from the measured overall surface impedance $Z$, we are able to extract and to comment on the London penetration depth, the flux flow resistivity and the pinning constant, highlighting the effect of artificial pinning centers in these samples.",1902.07589v1 2020-02-25,"Shear thickening and jamming of dense suspensions: the ""roll"" of friction","Particle-based simulations of discontinuous shear thickening (DST) and shear jamming (SJ) suspensions are used to study the role of stress-activated constraints, with an emphasis on resistance to gear-like rolling. Rolling friction decreases the volume fraction required for DST and SJ, in quantitative agreement with real-life suspensions with adhesive surface chemistries and ""rough"" particle shapes. It sets a distinct structure of the frictional force network compared to only sliding friction, and from a dynamical perspective leads to an increase in the velocity correlation length, in part responsible for the increased viscosity. The physics of rolling friction is thus a key element in achieving a comprehensive understanding of strongly shear-thickening materials.",2002.10996v2 2020-09-16,Superconductivity in CuAl2-type Co0.2Ni0.1Cu0.1Rh0.3Ir0.3Zr2 with a high-entropy-alloy transition metal site,"Research on high-entropy-alloy (HEA) superconductors is a growing field in material science. In this study, we explored new HEA-type superconductors and discovered a CuAl2-type superconductor Co0.2Ni0.1Cu0.1Rh0.3Ir0.3Zr2 with a HEA-type transition metal site. A superconducting transition was observed at 8.0 K after electrical resistivity, magnetization, and specific heat measurements. The bulk characteristics of the superconductivity were confirmed through the specific heat measurements. The discovery of superconductivity in HEA-type Co0.2Ni0.1Cu0.1Rh0.3Ir0.3Zr2 will provide a novel pathway to explore new HEA-type superconductors and investigate the relationship between the mixing entropy and superconductivity of HEA-type compounds.",2009.07548v3 2017-05-17,High Thermoelectric Figure of Merit by Resonant Dopant in Half-Heusler Alloys,"Half-Heusler alloys have been one of the benchmark high temperature thermoelectric materials owing to their thermal stability and promising figure of merit ZT. Simonson et al. early showed that small amounts of vanadium doped in Hf0.75Zr0.25NiSn enhanced the Seebeck coefficient and correlated the change with the increased density of states near the Fermi level. We herein report a systematic study on the role of vanadium (V), niobium (Nb), and tantalum (Ta) as prospective resonant dopants in enhancing the ZT of n-type half-Heusler alloys based on Hf0.6Zr0.4NiSn0.995Sb0.005. The V doping was found to increase the Seebeck coefficient in the temperature range 300-1000 K, consistent with a resonant doping scheme. In contrast, Nb and Ta act as normal n-type dopants, as evident by the systematic decrease in electrical resistivity and Seebeck coefficient. The combination of enhanced Seebeck coefficient due to the presence of V resonant states and the reduced thermal conductivity has led to a state-of-the-art ZT of 1.3 near 850 K in n-type (Hf0.6Zr0.4)0.99V0.01NiSn0.995Sb0.005 alloys.",1705.06100v1 2019-03-12,Superconductivity behavior in epitaxial TiN films points at surface magnetic disorder,"We analyze the evolution of the normal and superconducting electronic properties in epitaxial TiN films, characterized by high Ioffe-Regel parameter values, as a function of the film thickness. As the film thickness decreases, we observe an increase of in the residual resistivity, which becomes dominated by diffusive surface scattering for $d\leq20\,$nm. At the same time, a substantial thickness-dependent reduction of the superconducting critical temperature is observed compared to the bulk TiN value. In such a high quality material films, this effect can be explained by a weak magnetic disorder residing in the surface layer with a characteristic magnetic defect density of $\sim10^{12}\,\mathrm{cm}^{-2}$. Our results suggest that surface magnetic disorder is generally present in oxidized TiN films.",1903.05009v3 2019-12-30,Pinning Dislocations in Colloidal Crystals with Active Particles that Seek Stacking Faults,"There is growing interest in functional, adaptive devices built from colloidal subunits of micron size or smaller. A colloidal material with dynamic mechanical properties could facilitate such microrobotic machines. Here we study via computer simulation how active interstitial particles in small quantities can be used to modify the bulk mechanical properties of a colloidal crystal. Passive interstitial particles are known to pin dislocations in metals, thereby increasing resistance to plastic deformation. We extend this tactic by employing anisotropic active interstitials that travel super-diffusively and bind strongly to stacking faults associated with partial dislocations. We find that: 1) interstitials that are effective at reducing plasticity compromise between strong binding to stacking faults and high mobility in the crystal bulk. 2) Reorientation of active interstitials in the crystal depends upon rotational transitions between high-symmetry crystal directions. 3) The addition of certain active interstitial shapes at concentrations as low as $60$ per million host particles ($0.006\%$) can create a shear threshold for dislocation migration.",1912.12792v1 2015-06-16,Correlation of Crystal Quality and Extreme Magnetoresistance of WTe$_2$,"High quality single crystals of WTe$_2$ were grown using a Te flux followed by a cleaning step involving self-vapor transport. The method is reproducible and yields consistently higher quality single crystals than are typically obtained via halide assisted vapor transport methods. Magnetoresistance (MR)values at 9 Tesla and 2 Kelvin as high as 1.75 million \%, nearly an order of magnitude higher than previously reported for this material, were obtained on crystals with residual resistivity ratio (RRR) of approximately 1250. The MR follows a near B$^2$ law (B = 1.95(1)) and, assuming a semiclassical model, the average carrier mobility for the highest quality crystal was found to be ~167,000 cm$^2$/Vs at 2 K. A correlation of RRR, MR ratio and average carrier mobility ($\mu_{avg}$) is found with the cooling rate during the flux growth.",1506.04823v1 2018-12-18,The role of β-titanium ligaments in the deformation of dual phase titanium alloys,"Multiphase titanium alloys are critical materials in high value engineering components, for instance in aero engines. Microstructural complexity is exploited through interface engineering during mechanical processing to realise significant improvements in fatigue and fracture resistance and strength. In this work, we explore the role of select interfaces using in-situ micromechanical testing with concurrent observations from high angular resolution electron backscatter diffraction (HR-EBSD). Our results are supported with post mortem transmission electron microscopy (TEM). Using micro-pillar compression, we performed in-depth analysis of the role of select {\beta}-titanium (body centred cubic) ligaments which separate neighbouring {\alpha}-titanium (hexagonal close packed) regions and inhibit the dislocation motion and impact strength during mechanical deformation. These results shed light on the strengthening mechanisms and those that can lead to strain localisation during fatigue and failure.",1812.07250v2 2019-10-14,Investigation of nitrogen polar p-type doped GaN/AlxGa(1-x)N superlattices for applications in wide-bandgap p-type field effect transistors,"In this study the MOCVD growth and electrical properties of N-polar modulation doped p-AlGaN/GaN superlattices (SLs) were investigated. Hole sheet charge density and mobility were studied as a function of the concentration of the p-type dopant Mg in the SL and the number of SL periods. Room temperature Hall measurements were carried out to determine the hole mobility and the sheet charge density. While the hole density increased with increasing number of SL periods, the hole mobility was largely unaffected.Hole mobilities as high as 18cm2/Vs at a simultaneous high hole density of 6.5e13 cm-2 were observed for N-polar SLs with a Mg modulation doping of 7.5e18 cm-3. For comparable uniformly doped Ga-polar SL samples, a mobility of 11cm2/Vs was measured. Lowest sheet resistance in the GaN/AlGaN materials system of 5kOhm/sq is also reported. Test-structure transistors were also fabricated to investigate the applicability of these SL structures, with planar device resulting in a current of 5mA/mm, and a FinFET structure resulting in a current of over 100mA/mm.",1910.06421v1 2019-11-27,Enhancement of the electronic thermoelectric properties of bulk strained silicon-germanium alloys using the scattering relaxation times from first principles,"We use first-principles electronic structure methods to calculate the electronic thermoelectric properties (i.e. due to electronic transport only) of single-crystalline bulk $n$-type silicon-germanium alloys vs Ge composition, temperature, doping concentration and strain. We find excellent agreement to available experiments for the resistivity, mobility and Seebeck coefficient. These results are combined with the experimental lattice thermal conductivity to calculate the thermoelectric figure of merit $ZT$, finding very good agreement with experiment. We predict that 3% tensile hydrostatic strain enhances the $n$-type $ZT$ by 50% at carrier concentrations of $n=10^{20}$ cm$^{-3}$ and temperature of $T=1200K$. These enhancements occur at different alloy compositions due to different effects: at 50% Ge composition the enhancements are achieved by a strain induced decrease in the Lorenz number, while the power factor remains unchanged. These characteristics are important for highly doped and high temperature materials, in which up to 50% of the heat is carried by electrons. At 70% Ge the increase in $ZT$ is due to a large increase in electrical conductivity produced by populating the high mobility $\Gamma$ conduction band valley, lowered in energy by strain.",1911.12149v1 2020-10-01,High magnetic field spin-valley-split Shubnikov-de Haas oscillations in a WSe$_2$ monolayer,"We study Shubnikov-de Haas oscillations in a p-type WSe$_2$ monolayer under very high magnetic field. The oscillation pattern is complex due to a large spin and valley splitting, in the non-fully-resolved Landau level regime. Our experimental data can be reproduced with a model in which the main parameter is the ratio between the Zeeman energy and the cyclotron energy. The model takes into account the Landau levels from both valleys with the same Gaussian broadening, which allows to predict the relative amplitude of the resistance oscillation originating from each valley. The Zeeman energy is found to be several times larger than the cyclotron energy. It translates into a large and increasing effective Land\'e factor as the hole density decreases, in the continuity of the values reported in the literature at lower carrier density.",2010.00510v1 2020-11-27,High-pressure effects on superconducting properties and crystal structure of Bi-based layered superconductor La2O2Bi3Ag0.6Sn0.4S6,"The effects of pressure on the superconducting properties of a Bi-based layered superconductor La2O2Bi3Ag0.6Sn0.4S6, which possesses a four-layer-type conducting layer, have been studied through the electrical resistance and magnetic susceptibility measurements. The crystal structure under pressure was examined using synchrotron X-ray diffraction at SPring-8. In the low-pressure regime, bulk superconductivity with a transition temperature Tc of ~ 4.5 K was induced by pressure, which was achieved by in-plane chemical pressure effect owing to the compression of the tetragonal structure. In the high-pressure regime above 6.4 GPa, a structural symmetry lowering was observed, and superconducting transitions with a Tc ~ 8 K were observed. Our results suggest the possible commonality on the factor essential for Tc in Bi-based superconductors with two-layer-type and four-layer-type conducting layers.",2011.13532v1 2021-02-01,Liquefaction-induced Plasticity from Entropy-boosted Amorphous Ceramics,"Ceramics are easy to break, and very few generic mechanisms are available for improving their mechanical properties, e.g., the 1975-discovered anti-fracture mechanism is strictly limited to zirconia and hafnia. Here we report a general mechanism for achieving high plasticity through liquefaction of ceramics. We further disclose the general material design strategies to achieve this difficult task through entropy-boosted amorphous ceramics (EBACs), enabling fracture-resistant properties that can withstand severe plastic deformation (e.g., over 95%, deformed to a thickness of a few nanometers) while maintaining high hardness and reduced modulus. The findings reported here open a new route to ductile ceramics and many applications.",2102.00802v1 2021-02-13,Mechanical Performance of 3D Printed Interpenetrating Phase Composites with Spinodal Topologies,"The mechanical response of interpenetrating phase composites (IPCs) with stochastic spinodal topologies is investigated experimentally and numerically. Model polymeric systems are fabricated by Polyjet multi-material printing, with the reinforcing phase taking the topology of a spinodal shell, and the remaining volume filled by a softer matrix. We show that spinodal shell IPCs have comparable compressive strength and stiffness to IPCs with two well-established periodic reinforcements, the Schwarz P triply periodic minimal surface (TPMS) and the octet truss-lattice, while exhibiting far less catastrophic failure and greater damage resistance, particularly at high volume fraction of reinforcing phase. The combination of high stiffness and strength and a long flat plateau after yielding makes spinodal shell IPCs a promising candidate for energy absorption and impact protection applications, where the lack of material softening upon large compressive strains can prevent sudden collapse. Importantly, in contrast with all IPCs with periodic reinforcements, spinodal shell IPCs are amenable to scalable manufacturing via self-assembly techniques.",2102.06707v1 2021-07-22,Anomalous High-Field Magnetotransport in CaFeAsF due to the Quantum Hall Effect,"CaFeAsF is an iron-based superconductor parent compound whose Fermi surface is quasi-two dimensional, composed of Dirac-electron and Schr\""odinger-hole cylinders elongated along the $c$ axis. We measured the longitudinal and Hall resistivities in CaFeAsF with the electrical current in the $ab$ plane in magnetic fields up to 45 T applied along the $c$ axis and obtained the corresponding conductivities via tensor inversion. We found that both the longitudinal and Hall conductivities approached zero above $\sim$40 T as the temperature was lowered to 0.4 K. Our analysis indicates that the Landau-level filling factor is $\nu$ = 2 for both electrons and holes at these high field strengths, resulting in a total filling factor $\nu$ = $\nu_{hole} - \nu_{electron}$ = 0. We therefore argue that the $\nu$ = 0 quantum Hall state emerges under these conditions.",2107.10460v4 2022-01-08,Atomic disorder and Berry phase driven anomalous Hall effect in Co2FeAl Heusler compound,"Co2-based Heusler compounds are the promising materials for the spintronics application due to their high Curie temperature, large spin-polarization, large magnetization density, and exotic transport properties. In the present manuscript, we report the anomalous Hall effect (AHE) in a polycrystalline Co2FeAl Heusler compound using combined experimental and theoretical studies. The Rietveld analysis of high-resolution synchrotron x-ray diffraction data reveals a large degree (~50 %) of antisite disorder between Fe and Al atoms. The analysis of anomalous transport data provides the experimental anomalous Hall conductivity (AHC) about 227 S/cm at 2 K with an intrinsic contribution of 155 S/cm, which has nearly constant variation with temperature. The detailed scaling analysis of anomalous Hall resistivity suggests that the AHE in Co2FeAl is governed by the Berry phase driven intrinsic mechanism. Our theoretical calculations reveal that the disorder present in Co2FeAl compound enhances the Berry curvature induced intrinsic AHC.",2201.02864v1 2022-07-15,High power density energy harvesting devices based on the anomalous Nernst effect of Co/Pt magnetic multilayers,"The anomalous Nernst effect (ANE) is a thermomagnetic phenomenon with potential applications in thermal energy harvesting. While many recent works studied the approaches to increase the ANE coefficient of materials, relatively little effort was devoted to increasing the power supplied by the effect. Here we demonstrate a nanofabricated device with record power density generated by the ANE. To accomplish this, we fabricate micrometer-sized devices in which the thermal gradient is three orders of magnitude higher than conventional macroscopic devices. In addition, we use Co/Pt multilayers, a system characterized by a high ANE thermopower (~1 microV/K), low electrical resistivity, and perpendicular magnetic anisotropy. These innovations allow us to obtain power densities of around 13 W/cm3. We believe that this design may find uses in harvesting wasted energy in e.g. electronic devices.",2207.07526v2 2023-02-20,A High Throughput Aqueous Passivation Testing Methodology for Compositionally Complex Alloys using Scanning Droplet Cell,"Compositionally complex alloy systems containing more than five principal elements allow exploring a wide range of compositions, processing, and structural variables with the hope for identifying unique properties. Such opportunities also apply to designing materials for improved corrosion resistance, regulated by a self-healing passive film. Such a rich landscape in reactivity and protectivity demands the search for high-throughput experimental testing workflows to uncover key metrics, indicative of superior properties. In this communication, one such methodology is demonstrated for evaluating passivation performance of a combinatorial library of Al0.7-x-yCoxCryFe0.15Ni0.15 thin film alloys in deaerated 0.1 mol/L H2SO4(aq), using a scanning droplet cell.",2302.09804v4 2023-09-29,Transforming Materials Discovery for Artificial Photosynthesis: High-Throughput Screening of Earth-Abundant Semiconductors,"We present a highly efficient workflow for designing semiconductor structures with specific physical properties, which can be utilized for a range of applications, including photocatalytic water splitting. Our algorithm generates candidate structures composed of earth-abundant elements that exhibit optimal light-trapping, high efficiency in \ce{H2} and/or \ce{O2} production, and resistance to reduction and oxidation in aqueous media. To achieve this, we use an ionic translation model trained on the Inorganic Crystal Structure Database (ICSD) to predict over thirty thousand undiscovered semiconductor compositions. These predictions are then screened for redox stability under Hydrogen Evolution Reaction (HER) or Oxygen Evolution Reaction (OER) conditions before generating thermodynamically stable crystal structures and calculating accurate band gap values for the compounds. Our approach results in the identification of dozens of promising semiconductor candidates with ideal properties for artificial photosynthesis, offering a significant advancement toward the conversion of sunlight into chemical fuels.",2310.00118v1 2023-10-28,Ultralong-term high-density data storage with atomic defects in SiC,"There is an urgent need to increase the global data storage capacity, as current approaches lag behind the exponential growth of data generation driven by the Internet, social media and cloud technologies. In addition to increasing storage density, new solutions should provide long-term data archiving that goes far beyond traditional magnetic memory, optical disks and solid-state drives. Here, we propose a concept of energy-efficient, ultralong, high-density data archiving based on optically active atomic-size defects in a radiation resistance material, silicon carbide (SiC). The information is written in these defects by focused ion beams and read using photoluminescence or cathodoluminescence. The temperature-dependent deactivation of these defects suggests a retention time minimum over a few generations under ambient conditions. With near-infrared laser excitation, grayscale encoding and multi-layer data storage, the areal density corresponds to that of Blu-ray discs. Furthermore, we demonstrate that the areal density limitation of conventional optical data storage media due to the light diffraction can be overcome by focused electron-beam excitation.",2310.18843v1 2003-04-30,Pulsed Laser Deposition of epitaxial titanium diboride thin films,"Epitaxial titanium diboride thin films have been deposited on sapphire substrates by Pulsed Laser Ablation technique. Structural properties of the films have been studied during the growth by Reflection High Energy Electron Diffraction (RHEED) and ex-situ by means of X-ray diffraction techniques; both kinds of measurements indicate a good crystallographic orientation of the TiB2 film both in plane and along the c axis. A flat surface has been observed by Atomic Force Microscopy imaging. Electrical resistivity at room temperature resulted to be five times higher than the value reported for single crystals. The films resulted to be also very stable at high temperature, which is very promising for using this material as a buffer layer in the growth of magnesium diboride thin films.",0304680v1 2016-02-19,Magnetic anisotropy of large floating-zone-grown single-crystals of SrRuO3,"SrRuO3 is a highly interesting material due to its anomalous-metal properties related with ferromagnetism and its relevance as conductive perovskite layer or substrate in heterostructure devices. We have used optical floating zone technique in an infrared image furnace to grow large single crystals of SrRuO3 with volumes attaining several hundred mm3. Crystals obtained for optimized growth parameters exhibit a high ferromagnetic Curie temperature of 165 K and a low-temperature magnetization of 1.6 muB at a magnetic field of 6 T. The high quality of the crystals is further documented by large residual resistance ratios of 75 and by crystal structure and chemical analyzes. With these crystals the magnetic anisotropy could be determined.",1602.06171v2 2014-08-11,High spin polarization in CoFeMnGe quaternary Heusler alloy,"We report the structure, magnetic property and spin polarization of CoFeMnGe equiatomic quaternary Heusler alloy. The alloy was found to exist in the L21 structure with considerable amount of DO3 disorder. Thermal analysis result indicated the Curie temperature is about 711K without any other phase transformation up to melting temperature. The magnetization value was close to that predicted by the Slater-Pauling curve. Current spin polarization of P = 0.70 {plus/minus}0.1 was deduced using point contact Andreev reflection (PCAR) measurements. Half-metallic trend in the resistivity has also been observed in the temperature range of 5 K to 300 K. Considering the high spin polarization and Curie temperature, this material appears to be promising for spintronic applications.",1408.2408v2 2019-04-01,Quantum transport in high-quality shallow InSb quantum wells,"InSb is one of the promising candidates to realize a topological state through proximity induced superconductivity in a material with strong spin-orbit interactions. In two-dimensional systems, thin barriers are needed to allow strong coupling between superconductors and semiconductors. However, it is still challenging to obtain a high-quality InSb two-dimensional electron gas in quantum wells close to the surface. Here we report on a molecular beam epitaxy grown heterostructure of InSb quantum wells with substrate-side Si-doping and ultra-thin InAlSb (5 nm, 25 nm, and 50 nm) barriers to the surface. We demonstrate that the carrier densities in these quantum wells are gate-tunable and electron mobilities up to 350,000 $\rm{cm^2(Vs)^{-1}}$ are extracted from magneto-transport measurements. Furthermore, from temperature-dependent magneto-resistance measurements, we extract an effective mass of 0.02 $m_0$ and find a Zeeman splitting compatible with the expected g-factor.",1904.00828v2 2021-06-28,Topological Anderson Insulator in cation-disordered Cu2ZnSnS4,"Abstract: Using ab initio calculations supported by experimental transport measurements, we present the first credible candidate for the realization of a disorder-induced Topological Anderson Insulator in a real material system. High energy reactive ball-milling produces a polymorph of Cu2ZnSnS4 with high cation disorder, which shows an inverted ordering of bands at the Brillouin zone center, in contrast to its ordered phase. Adiabatic continuity arguments establish that this disordered Cu2ZnSnS4 can be connected to the closely related Cu2ZnSnSe4, previously predicted to be a 3D topological insulator. Band structure calculations with a slab geometry reveal the presence of robust surface states, while impedance spectroscopy coupled with resistivity measurements point to the surface-dominated transport which such states would imply; thus making a strong case in favor of a novel topological phase. As such, this study opens up a window to understanding and potentially exploiting topological behavior in a rich class of easily-synthesized multinary, disordered compounds.",2106.14714v1 2023-12-11,"Impersonating a Superconductor: High-Pressure BaCoO$_3$, an Insulating Ferromagnet","We report the high-pressure synthesis (6 GPa, 1200 $^{\circ}$C) and ambient pressure characterization of hexagonal HP-BaCoO$_3$. The material (with the 2H crystal structure) has a short intrachain Co-Co distance of about 2.07 $\text{\r{A}}$. Our magnetization investigation revealed robust diamagnetic behavior below approximately 130 K when exposed to weak applied magnetic fields (10 Oe) and a distinct half-levitation phenomenon below that temperature, such as is often observed for superconductors. Its field-dependent magnetization profile, however, unveils the characteristics of ferromagnetism, marked by a substantial magnetic retentivity of 0.22(1) ${\mu}_B$/Co at a temperature of 2 K. Electrical resistivity measurements indicate that HP-BaCoO$_3$ is a ferromagnetic insulator, not a superconductor.",2312.14955v1 2022-10-03,The impact of resistive electric fields on particle acceleration in reconnection layers,"In the context of particle acceleration in high-energy astrophysical environments featuring magnetic reconnection, the importance of the resistive term of the electric field compared to the convective one is still under debate. In this work, we present a quantitative analysis through 2D magnetohydrodynamic numerical simulations of tearing-unstable current sheets coupled to a test-particles approach, performed with the PLUTO code. We find that the resistive field plays a significant role in the early-stage energization of high-energy particles. Indeed, these particles are firstly accelerated due to the resistive electric field when they cross an X-point, created during the fragmentation of the current sheet. If this preliminary particle acceleration mechanism dominated by the resistive field is neglected, particles cannot reach the same high energies. Our results support therefore the conclusion that the resistive field is not only non-negligible but it does actually play an important role in the particle acceleration mechanism.",2210.01113v1 2024-01-31,Investigation of Microstructure and Corrosion Resistance of Ti-Al-V Titanium Alloys Obtained by Spark Plasma Sintering,"The research results of the microstructure and corrosion resistance of Ti and Ti-Al-V Russian industrial titanium alloys obtained by spark plasma sintering (SPS) are described. Investigations of the microstructure, phase composition, hardness, tensile strength, electrochemical corrosion resistance and hot salt corrosion of Ti-Al-V titanium alloy specimens were carried out. It was shown that the alloy specimens have a uniform highly dense microstructure and high hardness values. The studied alloys also have high resistance to electrochemical corrosion during tests in acidic aqueous solution causing the intergranular corrosion as well as high resistance to the hot salt corrosion. The assumption that the high hardness of the alloys as well as the differences in the corrosion resistance of the central and lateral parts of the specimens are due to the diffusion of carbon from the graphite mold into the specimen surface was suggested.",2401.17941v1 2003-02-01,High-Temperature Hall Effect in Ga(1-x)Mn(x)As,"The temperature dependence of the Hall coefficient of a series of ferromagnetic Ga(1-x)Mn(x)As samples is measured in the temperature range 80K < T < 500K. We model the Hall coefficient assuming a magnetic susceptibility given by the Curie-Weiss law, a spontaneous Hall coefficient proportional to rho_xx^2(T), and including a constant diamagnetic contribution in the susceptibility. For all low resistivity samples this model provides excellent fits to the measured data up to T=380K and allows extraction of the hole concentration (p). The calculated p are compared to alternative methods of determining hole densities in these materials: pulsed high magnetic field (up to 55 Tesla) technique at low temperatures (less than the Curie temperature), and electrochemical capacitance- voltage profiling. We find that the Anomalous Hall Effect (AHE) contribution to rho_xy is substantial even well above the Curie temperature. Measurements of the Hall effect in this temperature regime can be used as a testing ground for theoretical descriptions of transport in these materials. We find that our data are consistent with recently published theories of the AHE, but they are inconsistent with theoretical models previously used to describe the AHE in conventional magnetic materials.",0302013v2 2007-06-15,Growth mechanisms and structure of fullerene-like carbon-based thin films: superelastic materials for tribological applications,"In this chapter we review our findings on the bonding structure and growth mechanisms of carbon-based thin solid films with fullerene-like (FL) microstructure. The so-called FL arrangements arise from the curvature and cross-linking of basal planes in graphitic-like structures, partially resembling that of molecular fullerenes. This three-dimensional superstructure takes advantage of the strength of planar pi bonds in sp2 hybrids and confers the material interesting mechanical properties, such as high hardness, high elastic recovery, low-friction and wear-resistance. These properties can be tailored by controlling the curvature, size and connectivity of the FL arrangements, making these materials promising coatings for tribological applications. We have focused our interest mostly on carbon nitride (CNx) since nitrogen promotes the formation of FL arrangements at low substrate temperatures and they are emerging over pure carbon coatings in tribological applications such as protective overcoats in magnetic hard disks. We address structural issues such as origin of plane curvature, nature of the cross-linking sites and sp2 clustering, together with growth mechanisms based on the role of film-forming precursors, chemical re-sputtering or concurrent ion assistance during growth.",0706.2258v1 2013-07-08,"Significant ZT Enhancement in p-type Ti(Co,Fe)Sb-InSb Nanocomposites via a Synergistic High Mobility Electron Injection Energy filtering and Boundary Scattering Approach","It has been demonstrated that InSb nanoinclusions, which are formed in situ, can simultaneously improve all three individual thermoelectric properties of the n-type half Heusler compound (Ti,Zr,Hf)(Co,Ni)Sb [Xie et al., Acta Mater. 58, 4795 (2010)]. In the work presented herein, we have adopted the same approach to the p-type half Heusler compound Ti(Co,Fe)Sb. The results of resistivity, Seebeck coefficient, thermal conductivity, and Hall coefficient measurements indicate that the combined high mobility electron injection, low energy electron filtering, and boundary scattering, again, lead to a simultaneous improvement of all three individual thermoelectric properties: enhanced Seebeck coefficient and electrical conductivity as well as reduced lattice thermal conductivity. A figure of merit of ZT=0.33 was attained at 900 K for the sample containing 1 atomic percent InSb nanoinclusions, a 450 percent improvement over the nanoinclusion-free sample. This represents a rare case that the same nanostructuring approach successfully works for both p-type and n-type thermoelectric materials of the same class, hence pointing to a promising materials design route for higher performance half-Heusler materials in the future and hopefully will realize similar improvement in TE devices based on such half Heusler alloys.",1307.2160v1 2018-06-21,Planar Hall effect in type II Dirac semimetal VAl$_{3}$,"The study of electronic properties in topological systems is one of the most fascinating topics in condensed matter physics, which has generated enormous interests in recent times. New materials are frequently being proposed and investigated to identify their non-trivial band structure. While sophisticated techniques such as angle-resolved photoemission spectroscopy have become popular to map the energy-momentum relation, the transport experiments lack any direct confirmation of Dirac and Weyl fermions in a system. From band structure calculations, VAl$_{3}$ has been proposed to be a type II topological Dirac semimetal. This material represents a large family of isostructural compounds, all having similar electronic band structure and is an ideal system to explore the rich physics of Lorentz symmetry violating Dirac fermions. In this work, we present a detailed analysis on the magnetotransport properties of VAl$_{3}$. A large, non-saturating magnetoresistance has been observed. Hall resistivity reveals the presence of two types of charge carriers with high mobility. Our measurements show a large planar Hall effect in this material, which is robust and can be easily detectable up to high temperature. This phenomenon originates from the relativistic chiral anomaly and non-trivial Berry curvature, which validates the theoretical prediction of the Dirac semimetal phase in VAl$_{3}$.",1806.08287v1 2017-08-17,Separation of Electron and Hole Dynamics in the Semimetal LaSb,"We report investigations on the magnetotransport in LaSb, which exhibits extremely large magnetoresistance (XMR). Foremost, we demonstrate that the resistivity plateau can be explained without invoking topological protection. We then determine the Fermi surface from Shubnikov - de Haas (SdH) quantum oscillation measurements and find good agreement with the bulk Fermi pockets derived from first principle calculations. Using a semiclassical theory and the experimentally determined Fermi pocket anisotropies, we quantitatively describe the orbital magnetoresistance, including its angle dependence. We show that the origin of XMR in LaSb lies in its high mobility with diminishing Hall effect, where the high mobility leads to a strong magnetic field dependence of the longitudinal magnetoconductance. Unlike a one-band material, when a system has two or more bands (Fermi pockets) with electron and hole carriers, the added conductance arising from the Hall effect is reduced, hence revealing the latent XMR enabled by the longitudinal magnetoconductance. With diminishing Hall effect, the magnetoresistivity is simply the inverse of the longitudinal magnetoconductivity, enabling the differentiation of the electron and hole contributions to the XMR, which varies with the strength and orientation of the magnetic field. This work demonstrates a convenient way to separate the dynamics of the charge carriers and to uncover the origin of XMR in multi-band materials with anisotropic Fermi surfaces. Our approach can be readily applied to other XMR materials.",1708.05416v2 2019-01-21,Solid-State Thermal Energy Storage Using Reversible Martensitic Transformations,"The identification and use of reversible Martensitic transformations, typically described as shape memory transformations, as a new class of solid-solid phase change material is experimentally demonstrated here for the first time. To prove this claim, time-domain thermoreflectance, frequency-domain thermoreflectance, and differential scanning calorimetry studies were conducted on commercial NiTi alloys to quantify thermal conductivity and latent heat. Additional Joule-heating experiments demonstrate successful temperature leveling during transient heating and cooling in a simulated environment. Compared to standard solid-solid materials and solid-liquid paraffin, these experimental results show that shape memory alloys provide up to a two order of magnitude higher Figure of Merit. Beyond these novel experimental results, a comprehensive review of >75 binary NiTi and NiTi-based ternary and quaternary alloys in the literature shows that shape memory alloys can be tuned in a wide range of transformation temperatures (from -50 to 330{deg}C), latent heats (from 9.1 to 35.1 J/g), and thermal conductivities (from 15.6 to 28 W/mK). This can be accomplished by changing the Ni and Ti balance, introducing trace elements, and/or by thermomechanical processing. Combining excellent corrosion resistance, formability, high strength and ductility, high thermal performance, and tunability, SMAs represent an exceptional phase change material that circumvents many of the scientific and engineering challenges hindering progress in this field.",1901.06990v1 2020-11-30,Discovery of carbon-based strongest and hardest amorphous material,"Carbon is likely the most fascinating element of the periodic table because of the diversity of its allotropes stemming from its variable (sp, sp2, and sp3) bonding motifs. Exploration of new forms of carbon has been an eternal theme of contemporary scientific research. Here we report on novel amorphous carbon phases containing high fraction of sp3 bonded atoms recovered after compressing fullerene C60 to previously unexplored high pressure and temperature. The synthesized carbons are the hardest and strongest amorphous materials known to date, capable of scratching diamond crystal and approaching its strength which is evidenced by complimentary mechanical tests. Photoluminescence and absorption spectra of the materials demonstrate they are semiconductors with tunable bandgaps in the range of 1.5-2.2 eV, comparable to that of amorphous silicon. A remarkable combination of the outstanding mechanical and electronic properties makes this class of amorphous carbons an excellent candidate for photovoltaic applications demanding ultrahigh strength and wear resistance.",2011.14819v2 2021-12-20,Ultrafast Multi-Shot Ablation and Defect Generation in Monolayer Transition Metal Dichalcogenides,"Transition metal dichalcogenides are known to possess large optical nonlinearities and driving these materials at high intensities is desirable for many applications. Understanding their optical responses under repetitive intense excitation is essential to improve the performance limit of these strong-field devices and to achieve efficient laser patterning. Here, we report the incubation study of monolayer MoS${}_{2}$ and WS${}_{2}$ induced by 160 fs, 800 nm pulses in air to examine how their ablation threshold scales with the number of admitted laser pulses. Both materials were shown to outperform graphene and most bulk materials; specifically, MoS${}_{2}$ is as resistant to radiation degradation as the best of the bulk thin films with a record fast saturation. Our modeling provides convincing evidence that the small reduction in threshold and fast saturation of MoS${}_{2}$ originates in its excellent bonding integrity against radiation-induced softening. Sub-ablation damages, in the forms of vacancies, lattice disorder, and nano-voids, were revealed by transmission electron microscopy, photoluminescence, Raman, and second harmonic generation studies, which were attributed to the observed incubation. For the first time, a sub-ablation damage threshold is identified for monolayer MoS${}_{2}$ to be 78% of single-shot ablation threshold, below which MoS${}_{2}$ remains intact for many laser pulses. Our results firmly establish MoS${}_{2}$ as a robust material for strong-field devices and for high-throughput laser patterning.",2112.10743v1 2024-03-19,Electrical transport crossover and large magnetoresistance in selenium deficient van der Waals HfSe2-x,"Transition metal dichalcogenides have received much attention in the past decade not only due to the new fundamental physics, but also due to the emergent applications in these materials. Currently chalcogenide deficiencies in TMDs are commonly believed either during the high temperature growth procedure or in the nanofabrication process resulting significant changes of their reported physical properties in the literature. Here we perform a systematic study involving pristine stochiometric HfSe2, Se deficient HfSe1.9 and HfSe1.8. Stochiometric HfSe2 transport results show semiconducting behavior with a gap of 1.1eV. Annealing HfSe2 under high vacuum at room temperature causes the Se loss resulting in HfSe1.9, which shows unconventionally large magnetoresistivity following the extended Kohler's rule at low temperatures below 50 K. Moreover, a clear electrical resistivity crossover, mimicking the metal-insulator transition, is observed in the HfSe1.9 single crystal. Further increasing the degree of deficiency in HfSe1.8 results in complete metallic electrical transport at all temperatures down to 2K. Such a drastic difference in the transport behaviors of stoichiometric and Se-deficient HfSe2 further emphasizes that defect control and engineering could be an effective method that could be used to tailor the electronic structure of 2D materials, potentially unlock new states of matter, or even discover new materials.",2403.12430v1 2018-09-27,Granular aluminum: A superconducting material for high impedance quantum circuits,"Superconducting quantum information processing machines are predominantly based on microwave circuits with relatively low characteristic impedance, of about 100 Ohm, and small anharmonicity, which can limit their coherence and logic gate fidelity. A promising alternative are circuits based on so-called superinductors, with characteristic impedances exceeding the resistance quantum $R_Q = 6.4$ k$\Omega$. However, previous implementations of superinductors, consisting of mesoscopic Josephson junction arrays, can introduce unintended nonlinearity or parasitic resonant modes in the qubit vicinity, degrading its coherence. Here we present a fluxonium qubit design using a granular aluminum (grAl) superinductor strip. Granular aluminum is a particularly attractive material, as it self-assembles into an effective junction array with a remarkably high kinetic inductance, and its fabrication can be in-situ integrated with standard aluminum circuit processing. The measured qubit coherence time $T_2^R$ up to 30 $\mu$s illustrates the potential of grAl for applications ranging from protected qubit designs to quantum limited amplifiers and detectors.",1809.10646v1 2012-11-29,Effects of Resistivity on Magnetized Core-Collapse Supernovae,"We studied roles of a turbulent resistivity in the core-collapse of a strongly magnetized massive star, carrying out 2D-resistive-MHD simulations. The three cases with different initial strengths of magnetic field and rotation are investigated; 1. strongly magnetized rotating core; 2.moderately magnetized rotating core; 3. very strongly magnetized non-rotating core. In each case, both an ideal-MHD model and resistive-MHD models are computed. As a result of computations, each model shows a matter eruption helped by a magnetic acceleration (and also by a centrifugal acceleration in the rotating cases). We found that a resistivity attenuates the explosion in case~1 and 2, while it enhances the explosion in case~3. We also found that in the rotating cases, main mechanisms for the amplification of a magnetic field in the post-bounce phase are an outward advection of magnetic field and a winding of poloidal magnetic field-lines by differential rotation, which are somewhat dampened down with the presence of a resistivity. Although the magnetorotational instability seems to occur in the rotating models, it will play only a minor role in a magnetic field amplification. Another impact of resistivity is that on the aspect ratio. In the rotating cases, a large aspect ratio of the ejected matters, $> 2.5$, attained in a ideal-MHD model is reduced to some extent in a resistive model. These results indicate that a resistivity possibly plays an important role in the dynamics of strongly magnetized supernovae.",1211.6817v2 2019-04-18,Scaling-up atomically thin coplanar semiconductor-metal circuitry via phase engineered chemical assembly,"Two-dimensional (2D) layered semiconductors, with their ultimate atomic thickness, have shown promise to scale down transistors for modern integrated circuitry. However, the electrical contacts that connect these materials with external bulky metals are usually unsatisfactory, which limits the transistor performance. Recently, contacting 2D semiconductors using coplanar 2D conductors has shown promise in reducing the problematic high resistance contacts. However, many of these methods are not ideal for scaled production. Here, we report on the large-scale, spatially controlled chemical assembly of the integrated 2H-MoTe2 field-effect transistors (FETs) with coplanar metallic 1T' MoTe2 contacts via phase engineered approaches. We demonstrate that the heterophase FETs exhibit ohmic contact behavior with low contact resistance, resulting from the coplanar seamless contact between 2H and 1T' MoTe2 confirmed by transmission electron microscopy characterizations. The average mobility of the heterophase FETs was measured to be as high as 23 cm2 V-1 s-1 (comparable with those of exfoliated single crystals), due to the large 2H MoTe2 single-crystalline domain (486{\mu}m). By developing a patterned growth method, we realize the 1T' MoTe2 gated heterophase FET array whose components of channel, gate, and contacts are all 2D materials. Finally, we transfer the heterophase device array onto a flexible substrate and demonstrate the near-infrared photoresponse with high photoresponsivity (~1.02 A/W). Our study provides a basis for the large-scale application of phase-engineered coplanar MoTe2 semiconductors-meter structure in advanced electronics and optoelectronics.",1904.08545v1 2023-09-27,High-Resolution Full-field Structural Microscopy of the Voltage Induced Filament Formation in Neuromorphic Devices,"Neuromorphic functionalities in memristive devices are commonly associated with the ability to electrically create local conductive pathways by resistive switching. The archetypal correlated material, VO2, has been intensively studied for its complex electronic and structural phase transition as well as its filament formation under applied voltages. Local structural studies of the filament behavior are often limited due to time-consuming rastering which makes impractical many experiments aimed at investigating large spatial areas or temporal dynamics associated with the electrical triggering of the phase transition. Utilizing Dark Field X-ray Microscopy (DFXM), a novel full-field x-ray imaging technique, we study this complex filament formation process in-operando in VO2 devices from a structural perspective. We show that prior to filament formation, there is a significant gain of the metallic rutile phase beneath the metal electrodes that define the device. We observed that the filament formation follows a preferential path determined by the nucleation sites within the device. These nucleation sites are predisposed to the phase transition and can persistently maintain the high-temperature rutile phase even after returning to room temperature, which can enable a novel training/learning mechanism. Filament formation also appears to follow a preferential path determined by a nucleation site within the device which is predisposed to the rutile transition even after returning to room temperature. Finally, we found that small isolated low-temperature phase clusters can be present inside the high-temperature filaments indicating that the filament structure is not uniform. Our results provide a unique perspective on the electrically induced filament formation in metal-insulator transition materials, which further the basic understanding of this resistive switching.",2309.15712v1 2020-12-23,"Separated transport relaxation scales and interband scattering in SrRuO$_3$, CaRuO$_3$, and Sr$_2$RuO$_4$ thin films","The anomalous charge transport observed in some strongly correlated metals raises questions as to the universal applicability of Landau Fermi liquid theory. The coherence temperature $T_{FL}$ for normal metals is usually taken to be the temperature below which $T^2$ is observed in the resistivity. Below this temperature, a Fermi liquid with well-defined quasiparticles is expected. However, metallic ruthenates in the Ruddlesden-Popper family, frequently show non-Drude low-energy optical conductivity and unusual $\omega/T$ scaling, despite the frequent observation of $T^2$ dc resistivity. Herein we report time-domain THz spectroscopy measurements of several different high-quality metallic ruthenate thin films and show that the optical conductivity can be interpreted in more conventional terms. In all materials, the conductivity has a two-Drude peak lineshape at low temperature and a crossover to a one-Drude peak lineshape at higher temperatures. The two-component low-temperature conductivity is indicative of two well-separated current relaxation rates for different conduction channels. We discuss three particular possibilities for the separation of rates: (a) Strongly energy-dependent inelastic scattering; (b) an almost-conserved pseudomomentum operator that overlaps with the current, giving rise to the narrower Drude peak; (c) the presence of multiple conduction channels that undergoes a crossover to stronger interband scattering at higher temperatures. None of these scenarios require the existence of exotic quasiparticles. The results may give insight into the possible significance of Hund's coupling in determining interband coupling in these materials. Our results also show a route towards understanding the violation of Matthiessen's rule in this class of materials and deviations from the ""Gurzhi"" scaling relations in Fermi liquids.",2012.12800v1 2016-05-09,An analytical model for the influence of contact resistance on thermoelectric efficiency,"An analytical model is presented that can account for both electrical and hot and cold thermal contact resistances when calculating the efficiency of a thermoelectric generator. The model is compared to a numerical model of a thermoelectric leg, for 16 different thermoelectric materials, as well as the analytical models of Ebling et. al. (2010) and Min \& Rowe (1992). The model presented here is shown to accurately calculate the efficiency for all systems and all contact resistances considered, with an average difference in efficiency between the numerical model and the analytical model of $-0.07\pm0.35$ pp. This makes the model more accurate than previously published models. The maximum absolute difference in efficiency between the analytical model and the numerical model is 1.14 pp for all materials and all contact resistances considered.",1605.03565v1 2017-12-22,Magnetoresistance in YBi and LuBi semimetals due to nearly perfect carrier compensation,"Monobismuthides of yttrium and lutetium are shown as new representatives of materials which exhibit extreme magnetoresistance and magnetic-field-induced resistivity plateau. At low temperatures and in magnetic field of 9T the magnetoresistance attains the order of magnitude of 10,000% and 1,000%, on YBi and LuBi, respectively. Our thorough examination of electron transport properties of both compounds show that observed features are the consequence of nearly perfect carrier compensation rather than of possible nontrivial topology of electronic states. The field-induced plateau of electrical resistivity can be explained with Kohler scaling. Anisotropic multi-band model of electronic transport describes very well the magnetic field dependence of electrical resistivity and Hall resistivity. Data obtained from the Shubnikov-de Haas oscillations analysis also confirm that Fermi surface of each compound contains almost equal amounts of holes and electrons. First-principle calculations of electronic band structure are in a very good agreement with the experimental data.",1712.08433v3 2020-05-07,Origin of the Significant Impact of Ta on the Creep Resistance of FeCrNi Alloys,"Heat resistant FeCrNi alloys are widely used in the petrochemical industry because they exhibit a unique combination of creep and oxidation resistance at temperatures exceeding 900$^\circ$C. Their creep properties are often optimized by micro-additions of carbide forming elements. In the present work, the influence of Ta micro-additions has been experimentally investigated both on as-cast and aged microstructures to understand the origin of the significant impact of this element on the creep resistance. Calculations with thermocal software were also carried out to support experimental data. It is shown that a small addition of Ta is beneficial as it increases the volume fraction of stable MC carbides. We demonstrate also that additions of Ta may have a dramatic effect on the thermal stability of microstructures. This is attributed to a smaller equilibrium volume fraction of M23C6 and more pronounced heterogeneous precipitation at MC/matrix interfaces. The influence on the creep properties in then discussed.",2005.03309v1 2022-10-07,Radiation-resistant aluminium alloy for space missions in the extreme environment of the solar system,"Future human-based exploration of our solar system requires the invention of materials that can resist harsh environments. Age-hardenable aluminium alloys would be attractive candidates for structural components in long-distance spacecrafts, but their radiation resistance to solar energetic particles is insufficient. Common hardening phases dissolve and displacement damage occurs in the alloy matrix, which strongly degrades properties. Here we present an alloy where hardening is achieved by T-phase, featuring a giant unit cell and highly-negative enthalpy of formation. The phase shows record radiation survivability and can stabilize an ultrafine-grained structure upon temperature and radiation in the alloy, therby successfully preventing displacement damage to occur. Such concept can be considered ideal for the next-generation space materials and the design of radiation resistant alloy.",2210.03397v3 2022-11-22,"Optical properties and corrosion resistance of Ti2AlC, Ti3AlC2, and Cr2AlC as candidates for Concentrated Solar Power receivers","New generation concentrated solar power (CSP) plants require new solar receiver materials with selective optical properties and excellent corrosion resistance against molten salts. MAX phases are promising materials for CSP applications due to their optical properties and resistance to thermal shocks. Herein, we report a solar absorptance >/= 0.5 and a thermal emittance of 0.17-0.31 between 600 and 1500 K for Cr2AlC, Ti2AlC, and Ti3AlC2. These compositions were also exposed to solar salt corrosion at 600{\deg}C for up to 4 weeks. Cr2AlC exhibited superior corrosion resistance due to the formation of a protective nanometric layer.",2211.12251v2 2020-01-16,Social Engineering Resistant 2FA,"Attackers increasingly, and with high success rates, use social engineering techniques to circumvent second factor authentication (2FA) technologies, compromise user accounts and sidestep fraud detection technologies. We introduce a social engineering resistant approach that we term device-aware 2FA, to replace the use of traditional security codes.",2001.06075v1 2019-01-12,Surface impedance measurements on Nb$_{3}$Sn at high magnetic fields,"Nb$_{3}$Sn is a superconductor of great relevance for perspective RF applications. We present for the first time surface impedance $Z_s$ measurements at 15 GHz and low RF field amplitude on Nb$_{3}$Sn in high magnetic fields up to 12 T, with the aim of increasing the knowledge of Nb$_{3}$Sn behavior in such conditions. $Z_s$ is a fundamental material parameter that directly gives useful information about the dissipative and reactive phenomena when the superconductor is subjected to high-frequency excitations. Therefore, we present an analysis of the measured $Z_s$ with the aim of extracting interesting data about pinning in Nb$_{3}$Sn at high frequencies. From $Z_s$ we extract the vortex motion complex resistivity to obtain the $r$-parameter and the depinning frequency $\nu_p$ in high magnetic fields. The comparison of the results with the literature shows that the measured $\nu_p$ on bulk Nb$_{3}$Sn is several times greater than that of pure Nb. This demonstrates how Nb$_{3}$Sn can be a good candidate for RF technological applications, also in high magnetic fields.",1901.03819v1 2020-08-25,Observation of High Harmonics of the Cyclotron Resonance in Microwave Transmission of a High-Mobility Two-Dimensional Electron System,"We report an observation of magnetooscillations of the microwave power transmitted through the high mobility two-dimensional electron system hosted by a GaAs quantum well. The oscillations reflect an enhanced absorption of radiation at high harmonics of the cyclotron resonance and follow simultaneously measured microwave-induced resistance oscillations (MIRO) in the dc transport. While the relative amplitude (up to 1%) of the transmittance oscillations appears to be small, they represent a significant (>50%) modulation of the absorption coefficient. The analysis of obtained results demonstrates that the low-B decay, magnitude, and polarization dependence of the transmittance oscillations accurately follow the theory describing photon-assisted scattering between distant disorder-broadened Landau levels. The extracted sample parameters reasonably well describe the concurrently measured MIRO. Our results provide an insight into the MIRO polarization immunity problem and pave the way to probe diverse high-frequency transport properties of high-mobility systems using precise transmission measurements.",2008.11114v1 2021-09-20,Giant anomalous Nernst signal in the antiferromagnet YbMnBi2,"Searching for a high anomalous Nernst effect (ANE) is crucial for thermoelectric energy conversion applications because the associated unique transverse geometry facilitates module fabrication. Topological ferromagnets with large Berry curvatures show high ANEs; however, they face drawbacks such as strong magnetic disturbances and low mobility due to high magnetization. Herein, we demonstrate that YbMnBi2, a canted antiferromagnet, has a large ANE conductivity of ~10 Am-1K-1 that surpasses the common high values (i.e. 3-5 Am-1K-1) observed so far in ferromagnets. The canted spin structure of Mn guarantees a nonzero Berry curvature but generates only a weak magnetization three orders of magnitude lower than that of general ferromagnets. The heavy Bi with a large spin-orbit coupling enables a high ANE and low thermal conductivity, whereas its highly dispersive px/y orbitals ensure low resistivity. The high anomalous transverse thermoelectric performance and extremely small magnetization makes YbMnBi2 an excellent candidate for transverse thermoelectrics.",2109.09382v1 2022-02-09,Low energy switching of phase change materials using a 2D thermal boundary layer,"The switchable optical and electrical properties of phase change materials (PCMs) are finding new applications beyond data storage in reconfigurable photonic devices. However, high power heat pulses are needed to melt-quench the material from crystalline to amorphous. This is especially true in silicon photonics, where the high thermal conductivity of the waveguide material makes heating the PCM energy inefficient. Here, we improve the energy efficiency of the laser-induced phase transitions by inserting a layer of two-dimensional (2D) material, either MoS2 or WS2, between the silica or silicon and the PCM. The 2D material reduces the required laser power by at least 40% during the amorphization (RESET) process, depending on the substrate. Thermal simulations confirm that both MoS2 and WS2 2D layers act as a thermal barrier, which efficiently confines energy within the PCM layer. Remarkably, the thermal insulation effect of the 2D layer is equivalent to a ~100 nm layer of SiO2. The high thermal boundary resistance induced by the van der Waals (vdW)-bonded layers limits the thermal diffusion through the layer interfaces. Hence, 2D materials with stable vdW interfaces can be used to improve the thermal efficiency of PCM-tuned Si photonic devices. Furthermore, our waveguide simulations show that the 2D layer does not affect the propagating mode in the Si waveguide, thus this simple additional thin film produces a substantial energy efficiency improvement without degrading the optical performance of the waveguide. Our findings pave the way for energy-efficient laser-induced structural phase transitions in PCM-based reconfigurable photonic devices.",2202.04699v1 2008-06-27,Electron pockets in the Fermi surface of hole-doped high-Tc superconductors,"High-temperature superconductivity occurs as copper oxides are chemically tuned to have a carrier concentration intermediate between their metallic state at high doping and their insulating state at zero doping. The underlying evolution of the electron system in the absence of superconductivity is still unclear and a question of central importance is whether it involves any intermediate phase with broken symmetry. The Fermi surface of underdoped YBa2Cu3Oy and YBa2Cu4O8 was recently shown to include small pockets in contrast with the large cylinder characteristic of the overdoped regime1, pointing to a topological change in the Fermi surface. Here we report the observation of a negative Hall resistance in the magnetic field-induced normal state of YBa2Cu3Oy and YBa2Cu4O8, which reveals that these pockets are electron-like. We propose that electron pockets arise most likely from a reconstruction of the Fermi surface caused by the onset of a density-wave phase, as is thought to occur in the electron-doped materials near the onset of antiferromagnetic order Comparison with materials of the La2CuO4 family that exhibit spin/charge density-wave order suggests that a Fermi surface reconstruction also occurs in those materials, pointing to a generic property of high-Tc superconductors.",0806.4621v1 2008-11-19,Elucidation of the origins of HTSC transport behaviour and quantum oscillations,"A detailed exposition is made of recent transport and 'quantum oscillation' results from HTSC systems covering the full range from overdoped to underdoped material. This now very extensive and high quality data set is interpreted here within the framework developed by the author of local pairs and boson-fermion resonance, arising in the context of negative-U behaviour in an inhomogeneous electronic environment. The strong inhomogeneity comes with the mixed-valent condition of these materials, which when underdoped lie in close proximity to the Mott-Anderson transition. The observed intense scattering is presented as resulting from pair formation and electron-boson collisions in the resonant crossover circumstance. The high level of scattering brings the systems to incoherence in the pseudogapped state, p < pc (= 0.183). In a high magnetic field the striped partition of the inhomogeneous charge distribution is much strengthened and regularized. Magnetization and resistance oscillations, of period dictated by the favoured positioning of the square fluxon array within the real space environment of the diagonal 2D charge striping array, are demonstrated to be responsible for the recently reported behaviour hitherto widely attributed to the quantum oscillation response of a much more standard Fermi liquid condition. A detailed analysis embracing all the experimental data serves to indicate that in the given conditions of very high field, low temperature, 2D-striped, underdoped, d-wave superconducting, HTSC material the flux quantum becomes doubled to h/e.",0811.3096v2 2011-11-04,Local Structure of the Superconductor K0.8Fe1.6+xSe2: Evidence of Large Structural Disorder,"The local structure of superconducting single crystals of K0.8Fe1.6+xSe2 with Tc = 32.6 K was studied by x-ray absorption spectroscopy. Near-edge spectra reveal that the average valence of Fe is 2+. The room temperature structure about the Fe, K and Se sites was examined by iron, selenium and potassium K-edge measurements. The structure about the Se and Fe sites shows a high degree of order in the nearest neighbor Fe-Se bonds. On the other hand, the combined Se and K local structure measurements reveal a very high level of structural disorder in the K layers. Temperature dependent measurements at the Fe sites show that the Fe-Se atomic correlation follows that of the Fe-As correlation in the superconductor LaFeAsO0.89F0.11 - having the same effective Einstein temperature (stiffness). In K0.8Fe1.6+xSe2, the nearest neighbor Fe-Fe bonds has a lower Einstein temperature and higher structural disorder than in LaFeAsO0.89F0.11. The moderate Fe site and high K site structural disorder is consistent with the high normal state resistivity seen in this class of materials. For higher shells, an enhancement of the second nearest neighbor Fe-Fe interaction is found just below Tc and suggests that correlations between Fe magnetic ion pairs beyond the first neighbor are important in models of magnetic order and superconductivity in these materials.",1111.1026v1 2017-02-14,Pressure-induced metallization and superconducting phase in ReS2,"Among the family of TMDs, ReS2 takes a special position, which crystalizes in a unique distorted low-symmetry structure at ambient conditions. The interlayer interaction in ReS2 is rather weak, thus its bulk properties are similar to that of monolayer. However, how does compression change its structure and electronic properties is unknown so far. Here using ab initio crystal structure searching techniques, we explore the high-pressure phase transitions of ReS2 extensively and predict two new high-pressure phases. The ambient pressure phase transforms to a ""distorted-1T"" structure at very low pressure and then to a tetragonal I41/amd structure at around 90 GPa. The ""distorted-1T"" structure undergoes a semiconductor-metal transition (SMT) at around 70 GPa with a band overlap mechanism. Electron-phonon calculations suggest that the I41/amd structure is superconducting and has a critical superconducting temperature of about 2 K at 100 GPa. We further perform high-pressure electrical resistance measurements up to 102 GPa. Our experiments confirm the SMT and the superconducting phase transition of ReS2 under high pressure. These experimental results are in good agreement with our theoretical predictions.",1702.04061v1 2018-05-04,Silicon Oxide Electron-Emitting Nanodiodes,"Electrically driven on-chip electron sources that do not need to be heated have been long pursued because the current thermionic electron sources show the problems of high power consumption, slow temporal response, bulky size, etc., but their realization remains challenging. Here we show that a nanogap formed by two electrodes on a silicon oxide substrate functions as an electron-emitting nanodiode after the silicon oxide in the nanogap is electrically switched to a high-resistance conducting state. A nanodiode based on graphene electrodes can be turned on by a voltage of ~7 V in ~100 ns and show an emission current of up to several microamperes, corresponding to an emission density of ~10^6 A cm^-2 and emission efficiency as high as 16.6%. We attribute the electron emission to be generated from a metal-insulator-metal tunneling diode on the substrate surface formed by the rupture of conducting filaments in silicon oxide. An array of 100 nanodiodes exhibits a global emission density of 5 A cm^-2 and stable emission with negligible current degradation over tens of hours under modest vacuum. The combined advantages of a low operating voltage, fast temporal response, high emission density and efficiency, convenient fabrication and integration, and stable emission in modest vacuum make silicon oxide electron-emitting nanodiodes a promising on-chip alternative to thermionic emission sources.",1805.01602v1 2019-11-04,Enhanced upper critical field in Co-doped Ba122 superconductors by lattice defect tuning,"Nanoscale defects in superconductors play a dominant role in enhancing superconducting properties through electron scattering, modulation of coherence length, and correlation with quantized magnetic flux. For iron-based superconductors (IBSCs) that are expected to be employed in high-field magnetic applications, a fundamental question is whether such defects develop an upper critical field (Hc2) similar to that of conventional BCS-type superconductors. Herein, we report the first demonstration of a significantly improved Hc2 in a 122-phase IBSC by introducing defects through high-energy milling. Co-doped Ba122 polycrystalline bulk samples (Ba(Fe,Co)2As2) were prepared by sintering powder which was partially mechanically alloyed through high-energy milling. A remarkable increase in full-width at half maximum of X-ray powder diffraction peaks, anomalous shrinkage in the a-axis, and elongation in the c-axis were observed. When lattice defects are introduced into the grains, semiconductor behavior of the electric resistivity at low temperature (T < 100 K), slight decrease in transition temperature (Tc), upturn of Hc2(T) near Tc, and a large increase in Hc2(T) slope were observed. The slope of Hc2(T) increased approximately by 50%, i.e., from 4 to 6 T/K, and exceeded that of single crystals and thin films. Defect engineering through high-energy milling is expected to facilitate new methods for the designing and tuning of Hc2 in 122-phase IBSCs.",1911.01080v1 2019-11-07,Chemical manipulation of hydrogen induced high p-type and n-type conductivity in Ga2O3,"Advancement of optoelectronic and high-power devices is tied to the development of wide band gap materials with excellent transport properties. However, bipolar doping (n-type and p-type doping) and realizing high carrier density while maintaining good mobility have been big challenges in wide band gap materials. Here P-type and n-type conductivity was introduced in beta-Ga2O3, an ultra-wide band gap oxide, by controlling hydrogen incorporation in the lattice without further doping. Hydrogen induced a 9-order of magnitude increase of n-type conductivity with donor ionization energy of 20 meV and resistivity of 10-4 Ohm.cm. The conductivity was switched to p-type with acceptor ionization energy of 42 meV by altering hydrogen incorporation in the lattice. Density functional theory calculations were used to examine hydrogen location in the Ga2O3 lattice and identified a new donor type as the source of this remarkable n-type conductivity. Positron annihilation spectroscopy confirmed this finding and the interpretation of the results. This work illustrates a new approach that allows a tunable and reversible way of modifying the conductivity of semiconductors and it is expected to have profound implications on semiconductor field. At the same time it demonstrates for the first time p-type and remarkable n-type conductivity in Ga2O3 which should usher in the development of Ga2O3 devices and advance optoelectronics and high-power devices",1911.02717v1 2021-03-01,Absence of magnetic evidence for superconductivity in hydrides under high pressure,"It is generally believed that magnetization measurements on sulfur hydride under high pressure performed in 2015 [1] provided ""final convincing evidence of superconductivity"" [2] in that material, in agreement with theoretical predictions [3,4]. Supported by this precedent, drops in resistance that were later observed in several other hydrides under high pressure [2,5] have been generally accepted as evidence of superconductivity without corroborating evidence from magnetic measurements. In this paper we challenge the original interpretation that the magnetic measurements on sulfur hydride performed in 2015 were evidence of superconductivity. We point out that a large paramagnetic contribution to the magnetic susceptibility was detected below Tc and argue that its temperature dependence rules out the possibility that it would be a background signal; instead the temperature dependence indicates that the paramagnetic behavior originated in the sample. We discuss possible explanations for this remarkable behavior and conclude that standard superconductors would not show such behavior. We also survey all the other published data from magnetic measurements on this class of materials and conclude that they do not provide strong evidence for superconductivity. Consequently, we call into question the generally accepted view that conventional superconductivity in hydrogen-rich materials at high temperature and pressure is a reality, and discuss the implications if it is not.",2103.00701v3 2021-08-15,"High power Figure-of-Merit, 10.6-kV AlGaN/GaN lateral Schottky barrier diode with single channel and sub-100-μm anode-to-cathode spacing","GaN-based lateral Schottky diodes (SBDs) have attracted great attention for high-power applications due to its combined high electron mobility and large critical breakdown field. However, the breakdown voltage (BV) of the SBDs are far from exploiting the material advantages of GaN at present, limiting the desire to use GaN for ultra-high voltage (UHV) applications. Then, a golden question is whether the excellent properties of GaN-based materials can be practically used in the UHV field? Here we demonstrate UHV AlGaN/GaN SBDs on sapphire with a BV of 10.6 kV, a specific on-resistance of 25.8 m{\Omega}.cm2, yielding a power figure of merit of more than 3.8 GW/cm2. These devices are designed with single channel and 85-{\mu}m anode-to-cathode spacing, without other additional electric field management, demonstrating its great potential for the UHV application in power electronics.",2108.06679v1 2023-11-14,A New Look at Calcium Digermanide CaGe$_2$: A High-Performing Semimetal Transparent Conducting Material for Ge Optoelectronics,"Following a recently manifested guide of how to team up infrared transparency and high electrical conductivity within semimetal materials [C. Cui $et$ $al.$ Prog. Mater. Sci. 2023, 136, 101112], we evaluate an applicability of the calcium digermanide (CaGe$_2$) thin film electrodes for the advanced Ge-based optical devices. Rigorous growth experiments were conducted to define the optimal annealing treatment and thickness of the Ca-Ge mixture for producing stable CaGe$_2$ layers with high figure of merit (FOM) as transparent conducting material. Ab-initio electronic band structure calculations and optical modeling confirmed CaGe$_2$ semimetal nature, which is responsible for a demonstrated high FOM. To test CaGe$_2$ electrodes under actual conditions, a planar Ge photodetector (PD) with metal-semiconductor-metal structure was fabricated, where CaGe$_2$/Ge interface acts as Schottky barrier. The resulting Ge PD with semimetal electrodes outperformed commercially available Ge devices in terms of both photoresponse magnitude and operated spectral range. Moreover, by using femtosecond-laser projection lithography, a mesh CaGe$_2$ electrode with the relative broadband transmittance of 90\% and sheet resistance of 20 $\Omega$/sq. was demonstrated, which further enhanced Ge PD photoresponse. Thus, obtained results suggest that CaGe$_2$ thin films have a great potential in numerous applications promoting the era of advanced Ge optoelectronics.",2311.07903v1 2023-12-14,"Unlocking High Performance, Ultra-Low Power Van der Waals Transistors: Towards Back-End-of-Line In-Sensor Machine Vision Applications","Recent reports on machine learning (ML) and machine vision (MV) devices have demonstrated the potentials of 2D materials and devices. Yet, scalable 2D devices are being challenged by contact resistance and Fermi Level Pinning (FLP), power consumption, and low-cost CMOS compatible lithography processes. To enable CMOS+2D, it is essential to find a proper lithography strategy that can fulfill these requirements. Here, we explore modified van der Waals (vdW) deposition lithography and demonstrate a relatively new class of van-der-Waals-Field-Effect-Transistors (vdW-FETs) based on 2D materials. This lithography strategy enables us to unlock high performance devices evident by high current on-off ratio (Ion/Ioff), high turn-on current density (Ion), and weak Fermi Level Pinning (FLP). We utilize this approach to demonstrate a gate-tunable near-ideal diode using MoS2/WSe2 heterojunction with an ideality factor of ~1.65 and current rectification of 102. We finally demonstrate a highly sensitive, scalable, and ultra-low power phototransistor using MoS2/ WSe2 vdW-FET for Back-End-of-Line (BEOL) integration. Our phototransistor exhibits the highest gate-tunable photoresponsivity achieved to date for white light detection with ultra-low power dissipation, enabling ultra-sensitive, ultra-fast, and efficient optoelectronic applications such as in-sensor neuromorphic machine vision. Our approach shows the great potential of modified vdW deposition lithography for back-end-of-line CMOS+2D applications.",2312.08634v1 2006-08-31,Systematic study of disorder induced by neutron irradiation in MgB2 thin films,"The effects of neutron irradiation on normal state and superconducting properties of epitaxial magnesium diboride thin films are studied up to fluences of 1020 cm-2. All the properties of the films change systematically upon irradiation. Critical temperature is suppressed and, at the highest fluence, no superconducting transition is observed down to 1.8 K. Residual resistivity progressively increases from 1 to 190 microohmcm; c axis expands and then saturates at the highest damage level. We discuss the mechanism of damage through the comparison with other damage procedures. The normal state magnetoresistivity of selected samples measured up to high fields (28 and 45T) allows to determine unambiguously the scattering rates in each band; the crossover between the clean and dirty limit in each sample can be monitored. This set of samples, with controlled amount of disorder, is suitable to study the puzzling problem of critical field in magnesium diboride thin films. The measured critical field values are extremely high (of the order of 50T in the parallel direction at low fluences) and turns out to be rather independent on the experimental resistivity, at least at low fluences. A simple model to explain this phenomenology is presented.",0608706v2 2001-11-30,Effects of Bulk and Surface Conductivity on the Performance of CdZnTe Pixel Detectors,"We studied the effects of bulk and surface conductivity on the performance of high-resistivity CdZnTe (CZT) pixel detectors with Pt contacts. We emphasize the difference in mechanisms of the bulk and surface conductivity as indicated by their different temperature behaviors. In addition, the existence of a thin (10-100 A) oxide layer on the surface of CZT, formed during the fabrication process, affects both bulk and surface leakage currents. We demonstrate that the measured I-V dependencies of bulk current can be explained by considering the CZT detector as a metal-semiconductor-metal system with two back-to-back Schottky-barrier contacts. The high surface leakage current is apparently due to the presence of a low-resistivity surface layer that has characteristics which differ considerably from those of the bulk material. This surface layer has a profound effect on the charge collection efficiency in detectors with multi-contact geometry; some fraction of the electric field lines originated on the cathode intersects the surface areas between the pixel contacts where the charge produced by an ionizing particle gets trapped. To overcome this effect we place a grid of thin electrodes between the pixel contacts; when the grid is negatively biased, the strong electric field in the gaps between the pixels forces the electrons landing on the surface to move toward the contacts, preventing the charge loss. We have investigated these effects by using CZT pixel detectors indium bump bonded to a custom-built VLSI readout chip.",0112001v1 2008-10-23,Thermopower across the pseudogap critical point of La(1.6-x)Nd(0.4)Sr(x)CuO(4): Evidence for a quantum critical point in a hole-doped high-Tc superconductor,"The thermopower S of the high-Tc superconductor La(1.6-x)Nd(0.4)Sr(x)CuO(4) was measured as a function of temperature T near its pseudogap critical point, the critical hole doping p* where the pseudogap temperature T* goes to zero. Just above p*, S/T varies as ln(1/T) over a decade of temperature. Below p*, S/T undergoes a large increase below T*. As with the temperature dependence of the resistivity, which is linear just above p* and undergoes a large upturn below T*, these are typical signatures of a quantum phase transition. This suggests that p* is a quantum critical point below which some order sets in, causing a reconstruction of the Fermi surface, whose fluctuations are presumably responsible for the linear-T resistivity and logarithmic thermopower. We discuss the possibility that this order is the ""stripe"" order known to exist in this material.",0810.4280v2 2009-09-23,Zooming on the Quantum Critical Point in Nd-LSCO,"Recent studies of the high-Tc superconductor La_(1.6-x)Nd_(0.4)Sr_(x)CuO_(4) (Nd-LSCO) have found a linear-T in-plane resistivity rho_(ab) and a logarithmic temperature dependence of the thermopower S / T at a hole doping p = 0.24, and a Fermi-surface reconstruction just below p = 0.24 [1, 2]. These are typical signatures of a quantum critical point (QCP). Here we report data on the c-axis resistivity rho_(c)(T) of Nd-LSCO measured as a function of temperature near this QCP, in a magnetic field large enough to entirely suppress superconductivity. Like rho_(ab), rho_(c) shows an upturn at low temperature, a signature of Fermi surface reconstruction caused by stripe order. Tracking the height of the upturn as it decreases with doping enables us to pin down the precise location of the QCP where stripe order ends, at p* = 0.235 +- 0.005. We propose that the temperature T_(rho) below which the upturn begins marks the onset of the pseudogap phase, found to be roughly twice as high as the stripe ordering temperature in this material.",0909.4218v1 2009-12-30,30 inch Roll-Based Production of High-Quality Graphene Films for Flexible Transparent Electrodes,"We report that 30-inch scale multiple roll-to-roll transfer and wet chemical doping considerably enhance the electrical properties of the graphene films grown on roll-type Cu substrates by chemical vapor deposition. The resulting graphene films shows a sheet resistance as low as ~30 Ohm/sq at ~90 % transparency which is superior to commercial transparent electrodes such as indium tin oxides (ITO). The monolayer of graphene shows sheet resistances as low as ~125 Ohm/sq with 97.4% optical transmittance and half-integer quantum Hall effect, indicating the high-quality of these graphene films. As a practical application, we also fabricated a touch screen panel device based on the graphene transparent electrodes, showing extraordinary mechanical and electrical performances.",0912.5485v3 2013-10-03,Aharonov-Bohm resistance magneto-oscillations on single-nanohole graphite and graphene structures,"Graphene is a stable single atomic layer material exhibiting two-dimensional electron gas of massless Dirac fermions of high mobility. One of the intriguing properties of graphene is a possibility of realization of the Tamm-type edge states. These states differ from the usual surface states caused by defects, impurities and other imperfections at the edge of the system, as well as they differ from the magnetic edge states caused by skipping cyclotron orbits. The Tamm states result from breaking of periodic crystal potential at the edge, they can exist even at zero magnetic field and form a conducting band. Until recently those states have been observed in graphene only by local STM technique and there were no direct experiments on their contribution to transport measurements. Here we present the experiments on Aharonov-Bohm (AB) oscillations of resistance in a single-nanohole graphite and graphene structures, it indicates the presence of conducting edge states cycling around nanohole. An estimation show the penetration depth of the edge states to be as short as about 2 nm. The oscillations persist up to temperature T=115 K and the T-range of their existence increases with a decrease of the nanohole diameter. The proposed mechanism of the AB oscillations based on the resonant intervalley backscattering of the Dirac fermions by the nanohole via the Tamm states. The experimental results are consistent with such a scenario. Our findings show a way towards interference devices operating at high temperatures on the edge states in graphene",1310.0991v1 2014-02-27,"Spin-charge interplay in antiferromagnetic La$_{2-x}$Sr$_{x}$CuO$_{4}$ studied by the muons, neutrons, and ARPES techniques","Exploring whether a spin density wave (SDW) is responsible for the charge excitations gap in the high-temperature superconducting cuprates is difficult, since the region of the phase diagram where the magnetic properties are clearly exposed is different from the region where the band dispersion is visible. On the one hand, long range magnetic order disappears as doping approaches 2% from below, hindering our ability to perform elastic neutron scattering (ENS). On the other hand, cuprates become insulating at low temperature when the doping approaches 2% from above, thus restricting angle-resolved photoemission spectroscopy (ARPES). In fact, ARPES data for samples with doping lower than 3% are rare and missing the quasiparticle peaks in the energy distribution curves (EDCs). The main problem is the high resistivity of extremely underdoped samples, which is detrimental to ARPES due to charging effects. Nevertheless, the resistivity of La$_{2-x}$Sr$_{x}$CuO$_{4}$ as a function of temperature, at 2% doping, has a broad minimum around 100K. This minimum opens a window for both experiments. By preparing a series of LSCO single crystals with $\sim $0.2-0.3% doping steps around 2%, we managed to find one to which both techniques apply. This allows us to explore the cross talk between the magnetic and electronic properties of the material.",1402.6936v1 2014-05-21,High Mobility WSe2 p- and n-Type Field Effect Transistors Contacted by Highly Doped Graphene for Low-Resistance Contacts,"We report the fabrication of both n-type and p-type WSe2 field effect transistors with hexagonal boron nitride passivated channels and ionic-liquid (IL)-gated graphene contacts. Our transport measurements reveal intrinsic channel properties including a metal-insulator transition at a characteristic conductivity close to the quantum conductance e2/h, a high ON/OFF ratio of >107 at 170 K, and large electron and hole mobility of ~200 cm2V-1s-1 at 160 K. Decreasing the temperature to 77 K increases mobility of electrons to ~330 cm2V-1s-1 and that of holes to ~270 cm2V-1s-1. We attribute our ability to observe the intrinsic, phonon limited conduction in both the electron and hole channels to the drastic reduction of the Schottky barriers between the channel and the graphene contact electrodes using IL gating. We elucidate this process by studying a Schottky diode consisting of a single graphene/WSe2 Schottky junction. Our results indicate the possibility to utilize chemically or electrostatically highly doped graphene for versatile, flexible and transparent low-resistance Ohmic contacts to a wide range of quasi-2D semiconductors. KEYWORDS: MoS2, WSe2, field-effect transistors, graphene, Schottky barrier, ionic-liquid gate",1405.5437v1 2015-01-07,Angle dependence of the orbital magnetoresistance in bismuth,"We present an extensive study of angle-dependent transverse magnetoresistance in bismuth, with a magnetic field perpendicular to the applied electric current and rotating in three distinct crystallographic planes. The observed angular oscillations are confronted with the expectations of semi-classic transport theory for a multi-valley system with anisotropic mobility and the agreement allows us to quantify the components of the mobility tensor for both electrons and holes. A quadratic temperature dependence is resolved. As Hartman argued long ago, this indicates that inelastic resistivity in bismuth is dominated by carrier-carrier scattering. At low temperature and high magnetic field, the threefold symmetry of the lattice is suddenly lost. Specifically, a $2\pi/3$ rotation of magnetic field around the trigonal axis modifies the amplitude of the magneto-resistance below a field-dependent temperature. By following the evolution of this anomaly as a function of temperature and magnetic field, we mapped the boundary in the (field, temperature) plane separating two electronic states. In the less-symmetric state, confined to low temperature and high magnetic field, the three Dirac valleys cease to be rotationally invariant. We discuss the possible origins of this spontaneous valley polarization, including a valley-nematic scenario.",1501.01584v2 2015-02-26,First principles design of divacancy defected graphene nanoribbon based rectifying and negative differential resistance device,"We have elaborately studied the electronic structure of 555-777 divacancy (DV) defected armchair edged graphene nanoribbon (AGNR) and transport properties of AGNR based two-terminal device constructed with one defected electrode and one N doped electrode, by using density functional theory and non-equilibrium Green's function based approach. The introduction of 555-777 DV defect into AGNRs, results in a shifting of the {\pi} and {\pi}* bands towards the higher energy value which indicates a shifting of the Fermi level towards the lower energy. Formation of a potential barrier, very similar to that of conventional p-n junction, has been observed across the junction of defected and N doped AGNR. The prominent asymmetric feature of the current in the positive and negative bias indicates the diode like property of the device with high rectifying efficiency within wide range of bias voltages. The device also shows robust negative differential resistance (NDR) with very high peak-to-valley ratio. The analysis of the shifting of the energy states of the electrodes and the modification of the transmission function with applied bias provides an insight into the nonlinearity and asymmetry observed in the I-V characteristics. Variation of the transport properties on the width of the ribbon has also been discussed.",1502.07465v1 2016-06-07,Superconductivity and Charge Density Wave in ZrTe$_{3-x}$Se$_{x}$,"Charge density wave (CDW), the periodic modulation of the electronic charge density, will open a gap on the Fermi surface that commonly leads to decreased or vanishing conductivity. On the other hand superconductivity, a commonly believed competing order, features a Fermi surface gap that results in infinite conductivity. Here we report that superconductivity emerges upon Se doping in CDW conductor ZrTe$_{3}$ when the long range CDW order is gradually suppressed. Superconducting critical temperature $T_c(x)$ in ZrTe$_{3-x}$Se$_x$ (${0\leq}x\leq0.1$) increases up to 4 K plateau for $0.04$$\leq$$x$$\leq$$0.07$. Further increase in Se content results in diminishing $T_{c}$ and filametary superconductivity. The CDW modes from Raman spectra are observed in $x$ = 0.04 and 0.1 crystals, where signature of ZrTe$_{3}$ CDW order in resistivity vanishes. The electronic-scattering for high $T_{c}$ crystals is dominated by local CDW fluctuations at high temperures, the resistivity is linear up to highest measured $T=300K$ and contributes to substantial in-plane anisotropy.",1606.02284v1 2016-07-15,Effect of interface on mid-infrared photothermal response of MoS2 thin film grown by pulsed laser deposition,"Here we report mid infrared (mid-IR) photothermal response of multi layer MoS2 thin film grown on crystalline (p-type silicon and c-axis oriented single crystal sapphire) and amorphous substrates (Si/SiO2 and Si/SiN) by pulsed laser deposition (PLD) technique. The photothermal response of the MoS2 films was measured as changes in the resistance of MoS2 films when irradiated with mid IR (7 to 8.2 {\mu}m) source. We show that it is possible to enhance the temperature coefficient of resistance (TCR) of the MoS2 thin film by controlling the interface through proper choice of substrate and growth conditions. The thin films grown by PLD were characterized using XRD, Raman, AFM, XPS and TEM. High-resolution transmission electron microscopy (HRTEM) images show that the MoS2 films grow on sapphire substrate in a layer-by-layer manner with misfit dislocations. Layer growth morphology is disrupted when grown on substrates with diamond cubic structure such as silicon due to growth twin formation. The growth morphology is very different on amorphous substrates such as Si/SiO2 or Si/SiN. The MoS2 film grown on silicon shows a very high TCR (-2.9% K-1), mid IR sensitivity (delR/R=5.2 %) and responsivity (8.7 V/W) as compared to films on other substrates.",1607.04682v1 2016-11-10,Pressure-induced quantum phase transition in the itinerant ferromagnet UCoGa,"In this paper, we report the results of a high pressure study of the itinerant 5f-electron ferromagnet UCoGa. The work is focused on probing the expected ferromagnet-to-paramagnet quantum phase transition induced by high pressure and on the general features of the P-T(-H) phase diagram. Diamond anvil cells were employed to measure the magnetization and electrical resistivity under pressures up to ~ 10 GPa.At ambient pressure, UCoGa exhibits collinear ferromagnetic ordering of uranium magnetic moments {\mu}U ~ 0.74 {\mu}B (at 2 K) aligned along the c-axis of the hexagonal crystal structure below Curie temperature TC = 48K. With the application of pressure, gradual decrease of both, TC and the saturated magnetic moment, has been observed up to pressures ~ 6 GPa. This is followed by a sharp drop of magnetic moment and a sudden disappearance of the magnetic order at the pressure of 6.5 GPa, suggesting a first-order phase transition, as expected for a clean system. The low temperature power law dependence of the electrical resistivity shows distinct anomalies around the ~ 6 GPa, consistent with the pressure evolution of the magnetic moment and the ordering temperature. The tricritical point of the UCoGa phase diagram is located at approximately ~ 30 K and ~ 6 GPa.",1611.03276v1 2016-11-14,Two-carrier analyses of the transport properties of black phosphorus under pressure,"We report on the electronic transport properties of black phosphorus and analyze them using a two-carrier model in a wide range of pressure up to 2.5 GPa. In semiconducting state at 0.29 GPa, the remarkable non-linear behavior in the Hall resistance is reasonably reproduced by assuming the coexistence of two kinds of hole with different densities and mobilities. On the other hand, two-carrier analyses of the magnetotransport properties above 1.01 GPa suggest the coexistence of high mobility electron and hole carriers that have almost the same densities, i.e., nearly compensated semimetallic nature of black phosphorus. In the semimetallic state, analyses of both the two-carrier model and quantum oscillations indicate a systematic increase in the carrier densities as pressure increases. An observed sign inversion of Hall resistivity at low magnetic fields suggests the existence of high mobility electrons (\sim105 cm2 V-1 s-1) that is roughly ten times larger than that of holes, in the semimetallic black phosphorus. We conclude that the extremely large positive magnetoresistance that has been observed in semimetallic state cannot be reproduced by a conventional two-carrier model.",1611.04277v2 2017-06-23,Fabrication of highly dense isotropic Nd-Fe-B bonded magnets via extrusion-based additive manufacturing,"Isotropic bonded magnets with a high loading fraction of 70 vol.% Nd-Fe-B are fabricated via an extrusion-based additive manufacturing, or 3D printing system that enables rapid production of large parts for the first time. The density of the printed magnet is 5.15 g/cm3. The room temperature magnetic properties are: intrinsic coercivity Hci = 8.9 kOe (708.2 kA/m), remanence Br = 5.8 kG (0.58 Tesla), and energy product (BH)max = 7.3 MGOe (58.1 kJ/m3). The as-printed magnets are then coated with two types of polymers, both of which improve the thermal stability at 127 {\deg}C as revealed by flux aging loss measurements. Tensile tests performed at 25 {\deg}C and 100 {\deg}C show that the ultimate tensile stress (UTS) increases with increasing loading fraction of the magnet powder, and decreases with increasing temperature. AC magnetic susceptibility and resistivity measurements show that the 3D printed Nd-Fe-B bonded magnets exhibit extremely low eddy current loss and high resistivity. Finally, we show that through back electromotive force measurements that motors installed with 3D printed Nd-Fe-B magnets exhibit similar performance as compared to those installed with sintered ferrites.",1706.07792v1 2017-10-11,Pressure Induced Superconductivity in the New Compound ScZrCo1-$δ$,"It is widely perceived that the correlation effect may play an important role in several unconventional superconducting families, such as cuprate, iron-based and heavy-fermion superconductors. The application of high pressure can tune the ground state properties and balance the localization and itineracy of electrons in correlated systems, which may trigger unconventional superconductivity. Moreover, non-centrosymmetric structure may induce the spin triplet pairing which is very rare in nature. Here, we report a new compound ScZrCo1-${\delta}$ crystallizing in the Ti2Ni structure with the space group of FD3-MS without a spatial inversion center. The resistivity of the material at ambient pressure shows a bad metal and weak semiconducting behavior. Furthermore, specific heat and magnetic susceptibility measurements yield a rather large value of Wilson ratio ~4.47. Both suggest a ground state with correlation effect. By applying pressure, the up-going behavior of resistivity in lowering temperature at ambient pressure is suppressed and gradually it becomes metallic. At a pressure of about 19.5 GPa superconductivity emerges. Up to 36.05 GPa, a superconducting transition at about 3.6 K with a quite high upper critical field is observed. Our discovery here provides a new platform for investigating the relationship between correlation effect and superconductivity.",1710.04047v1 2019-05-07,Nonsaturating magnetoresistance and nontrivial band topology of type-II Weyl semimetal NbIrTe4,"Weyl semimetals, characterized by nodal points in the bulk and Fermi arc states on the surface, have recently attracted extensive attention due to the potential application on low energy consumption electronic materials. In this report, the thermodynamic and transport properties of a theoretically predicted Weyl semimetal NbIrTe4 is measured in high magnetic fields up to 35 T and low temperatures down to 0.4 K. Remarkably, NbIrTe4 exhibits a nonsaturating transverse magnetoresistance which follows a power-law dependence in B. Low-field Hall measurements reveal that hole-like carriers dominate the transport for T $>$ 80 K, while the significant enhancement of electron mobilities with lowering T results in a non-negligible contribution from electron-like carriers which is responsible for the observed non-linear Hall resistivity at low T. The Shubnikov-de Haas oscillations of the Hall resistivity under high B give the light effective masses of charge carriers and the nontrivial Berry phase associated with Weyl fermions. Further first-principles calculations confirm the existence of 16 Weyl points located at kz = 0, $\pm$0.02 and $\pm$0.2 planes in the Brillouin zone.",1905.02455v1 2014-08-29,Exotic Kondo crossover in a wide temperature region in the topological Kondo insulator SmB6 revealed by high-resolution ARPES,"Temperature dependence of the electronic structure of SmB6 is studied by high-resolution ARPES down to 1 K. We demonstrate that there is no essential difference for the dispersions of the surface states below and above the resistivity saturating anomaly (~ 3.5 K). Quantitative analyses of the surface states indicate that the quasi-particle scattering rate increases linearly as a function of temperature and binding energy, which differs from Fermi-Liquid behavior. Most intriguingly, we observe that the hybridization between the d and f states builds gradually over a wide temperature region (30 K < T < 110 K). The surface states appear when the hybridization starts to develop. Our detailed temperature-dependence results give a complete interpretation of the exotic resistivity result of SmB6, as well as the discrepancies among experimental results concerning the temperature regions in which the topological surface states emerge and the Kondo gap opens, and give new insights into the exotic Kondo crossover and its relationship with the topological surface states in the topological Kondo insulator SmB6.",1408.7090v1 2018-10-08,Correlation between scale-invariant normal state resistivity and superconductivity in an electron-doped cuprate,"An understanding of the normal state in the high-temperature superconducting cuprates is crucial to the ultimate understanding of the long-standing problem of the origin of the superconductivity itself. This so-called strange metal state is thought to be associated with a quantum critical point (QCP) hidden beneath the superconductivity(1,2). In electron-doped cuprates in contrast to hole-doped cuprates it is possible to access the normal state at very low temperatures and low magnetic fields to study this putative QCP and to probe the T~0 K state of these materials(3,4). We report measurements of the low temperature normal state magnetoresistance (MR) of the n-type cuprate system La2-xCexCuO4 (LCCO) and find that it is characterized by a linear-in-field behavior, which follows a scaling relation with applied field and temperature, for doping (x) above the putative QCP (x= 0.14)(5). This unconventional behavior suggests that magnetic fields probe the same physics that gives rise to the anomalous low-temperature linear-in-T resistivity(4). The magnitude of the linear MR decreases as Tc decreases and goes to zero at the end of the superconducting dome (x ~0.175) above which a conventional quadratic MR is found. These results show that there is a strong correlation between the quantum critical excitations of the strange metal state and the high-Tc superconductivity.",1810.03499v1 2017-04-12,Fabrication of Simple Apparatus for Resistivity Measurement in High Temperature Range 300-620 K,"A simple and low cost apparatus has been designed and built to measure the electrical resistivity, ($\rho$), of metal and semiconductors in 300-620 K temperature range. The present design is suitable to do measurement on rectangular bar sample by using conventional four-probe dc method. A small heater is made on the sample mounting copper block to achieve the desired temperature. Heat loss from sample holder is minimize by using very low thermal conductive insulator block. This unique design of heater and minimized heat loss from sample platform provide uniform sample temperature and also have very good thermal stability during the measurement. The electrical contacts of current leads and potential probes on the sample are done by using very thin (42 SWG) copper wires and high temperature silver paste. The use of limited components and small heater design make present instrument very simple, light weight, easy to sample mount, small in size, and low cost. To calibrate the instrument pure nickel sample was used, and two other materials La$_{0.7}$Sr$_{0.3}$MnO$_{3}$ (LSMO) and LaCoO$_{3}$ (LCO) were also characterized to demonstrate the accuracy of this set-up. $\rho$(T) behavior on these samples were found to be in good agreement with the reported data. The metal-insulator transition for LSMO (T$_{MI}$ = $\sim$358 K) and the insulator-metal transition for LCO (T$_{IM}$ = $\sim$540 K) were clearly observed and these transitions temperature were also consistent with those reported in literature.",1704.04122v1 2019-03-15,Enhanced Tunnelling in a Hybrid of Single-Walled Carbon Nanotubes and Graphene,"Transparent and conductive films (TCFs) are of great technological importance. The high transmittance, electrical conductivity and mechanical strength make single-walled carbon nanotubes (SWCNTs) a good candidate for their raw material. Despite the ballistic transport in individual SWCNTs, however, the electrical conductivity of their networks is limited by low efficiency of charge tunneling between the tube elements. Here, we demonstrate that the nanotube network sheet resistance at high optical transmittance is decreased by more than 50% when fabricated on graphene and thus provides a comparable improvement as widely adopted gold chloride ($\mathrm{AuCl_3}$) doping. However, while Raman spectroscopy reveals substantial changes in spectral features of doped nanotubes, no similar effect is observed in presence of graphene. Instead, temperature dependent transport measurements indicate that graphene substrate reduces the tunneling barrier heights while its parallel conductivity contribution is almost negligible. Finally, we show that combining the graphene substrate and $\mathrm{AuCl_3}$ doping, the SWCNT thin films can exhibit sheet resistance as low as 36 $\Omega$/sq. at 90% transmittance.",1903.06449v1 2019-04-04,Anomalous high-magnetic field electronic state of the nematic superconductors FeSe$_{1-x}$S$_x$,"Understanding superconductivity requires detailed knowledge of the normal electronic state from which it emerges. A nematic electronic state that breaks the rotational symmetry of the lattice can potentially promote unique scattering relevant for superconductivity. Here, we investigate the normal transport of superconducting FeSe$_{1-x}$S$_x$ across a nematic phase transition using high magnetic fields up to 69 T to establish the temperature and field-dependencies. We find that the nematic state is an anomalous non-Fermi liquid, dominated by a linear resistivity at low temperatures that can transform into a Fermi liquid, depending on the composition $x$ and the impurity level. Near the nematic end point, we find an extended temperature regime with $T^{1.5}$ resistivity. The transverse magnetoresistance inside the nematic phase has as a $H^{1.55}$ dependence over a large magnetic field range and it displays an unusual peak at low temperatures inside the nematic phase. Our study reveals anomalous transport inside the nematic phase, driven by the subtle interplay between the changes in the electronic structure of a multi-band system and the unusual scattering processes affected by large magnetic fields and disorder",1904.02522v1 2019-08-13,Magnetization Current Simulation of High Temperature Bulk Superconductors Using A-V-A Formulation and Iterative Algorithm Method: Critical State Model and Flux Creep Model,"In this work we will introduce the A-V-A formulation based iterative algorithm method (IAM) for simulating the magnetization current of high temperature superconductors. This new method embedded in ANSYS can simulate the critical state model by forcing the trapped current density to the critical current density Jc for all meshed superconducting elements after each iterative load step, as well as simulate the flux creep model by updating the E-J power law based resistivity values. The simulation results of a disk-shaped ReBCO bulk during zero field cooling (ZFC) or field cooling (FC) magnetization agree well with the simulation results from using the H-formulation in COMSOL. The computation time is shortened by using the A-V formulation in superconductor areas and the A-formulation in non-superconductor areas. This iterative method is further proved friendly for adding ferromagnetic materials into the FEA model or taking into account the magnetic field-dependent or mechanical strain-related critical current density of the superconductors. The influence factors for the magnetization simulation, including the specified iterative load steps, the initial resistivity, the ramping time and the updating coefficient, are discussed in detail. The A-V-A formulation based IAM, implemented in ANSYS, shows its unique advantages in adjustable computation time, multi-frame restart analysis and easy-convergence.",1908.04640v2 2015-07-17,Study of the Effects of High-Energy Proton Beams on Escherichia Coli,"Antibiotic-resistant bacterial infection becomes one of the most serious risks to public health care today. However, discouragingly, the development of new antibiotics has been little progressed over the last decade. There is an urgent need of the alternative approaches to treat the antibiotic-resistant bacteria. The novel methods, which include photothermal therapy based on gold nano-materials and ionizing radiation such as X-rays and gamma rays, have been reported. Studies of the effects of high-energy proton radiation on bacteria are mainly focused on Bacillus species and its spores. The effect of proton beams on Escherichia coli (E. coli) has been limitedly reported. The Escherichia coli is an important biological tool to obtain the metabolic and genetic information and also a common model microorganism for studying toxicity and antimicrobial activity. In addition, E. coli is a common bacterium in the intestinal tract of mammals. Herein, the morphological and physiological changes of E. coli after proton irradiation were investigated. The diluted solutions of the cells were used for proton beam radiation. LB agar plates were used to count the number of colonies formed. The growing profile of the cells was monitored by optical density at 600 nm. The morphology of the irradiated cells was analyzed with optical microscope. Microarray analysis was performed to examine the gene expression changes between irradiated samples and control samples without irradiation.",1507.04863v1 2020-12-02,Incoherent transport across the strange metal regime of highly overdoped cuprates,"Strange metals possess highly unconventional transport characteristics, such as a linear-in-temperature ($T$) resistivity, an inverse Hall angle that varies as $T^2$ and a linear-in-field ($H$) magnetoresistance. Identifying the origin of these collective anomalies has proved profoundly challenging, even in materials such as the hole-doped cuprates that possess a simple band structure. The prevailing dogma is that strange metallicity in the cuprates is tied to a quantum critical point at a doping $p*$ inside the superconducting dome. Here, we study the high-field in-plane magnetoresistance of two superconducting cuprate families at doping levels beyond $p*$. At all dopings, the magnetoresistance exhibits quadrature scaling and becomes linear at high $H/T$ ratios. Moreover, its magnitude is found to be much larger than predicted by conventional theory and insensitive to both impurity scattering and magnetic field orientation. These observations, coupled with analysis of the zero-field and Hall resistivities, suggest that despite having a single band, the cuprate strange metal phase hosts two charge sectors, one containing coherent quasiparticles, the other scale-invariant `Planckian' dissipators.",2012.01208v2 2021-11-16,Orbital Selective Kondo Effect in Heavy Fermion Superconductor UTe$_{2}$,"It has been a great challenge to explore many-body effects in heavy fermion systems with $ab$-$initio$ approaches. We computed the electronic structure of UTe$_{2}$ without purposive judgements, such as intentional selection of on-site Coulomb interaction and disregarding spin-orbit coupling. We show that U-5$f$ electrons are highly localized in the paramagnetic normal state, giving rise to the Kondo effect. It is also found that the hybridization between U-5$f$ and U-6$d$ predominantly in the orthorhombic $ab$-plane is responsible for the high-temperature Kondo effect. In contrast, the hybridization between U-5$f$ and Te-5$p$ along the $c$-axis manifests the Kondo scattering at a much lower temperature, which could be responsible for the low-temperature upturn of the $c$-axis resistivity. Our results show that the electron correlation in UTe$_2$ is orbital selective, which naturally elucidates the recent experimental observations of anomalous temperature dependence of resistivity. Furthermore, we suggest that the Kondo effect is suppressed at high pressure owing to weak localization of magnetic moments, which results from enhanced U-5$f$ electron hopping.",2111.08800v4 2022-07-10,Engineering underdoped CuO$_2$ nanoribbons in nm-thick $a$-axis YBa$_2$Cu$_3$O$_{7-δ}$ films,"In underdoped cuprate high $T_{\mathrm{c}}$ superconductors, various local orders and symmetry breaking states, in addition to superconductivity, reside in the CuO$_2$ planes. The confinement of the CuO$_2$ planes can therefore play a fundamental role in modifying the hierarchy between the various orders and their intertwining with superconductivity. Here we present the growth of $a$-axis oriented YBa$_2$Cu$_3$O$_{7-\delta}$ films, spanning the whole underdoped side of the phase diagram. In these samples, the CuO$_2$ planes are confined by the film thickness, effectively forming unit-cell-thick nanoribbons. The unidirectional confinement at the nanoscale enhances the in-plane anisotropy of the films. By X-ray diffraction and resistance vs temperature measurements, we have discovered the suppression of the orthorhombic-to-tetragonal transition at low dopings, and a very high anisotropy of the normal state resistance in the $b$-$c$ plane, the latter being connected to a weak coupling between adjacent CuO$_2$ nanoribbons. These findings show that the samples we have grown represent a novel system, different from the bulk, where future experiments can possibly shed light on the rich and mysterious physics occurring within the CuO$_2$ planes.",2207.04541v3 2022-12-11,Strain induced variations in transport and optical properties of SrVO$_3$: a DFT+U study,"First-principles calculations based on density functional theory + Hubbard U (DFT+U) approach have been carried out to study the strain induced variations in the optical and transport properties of the correlated perovskite SrVO$_3$. By virtue of its conductivity, high carrier mobility and optical transparency, SrVO$_3$ can be used as a potential replacement of indium tin oxide (ITO) as a transparent conductor. As strain tuning is an effective way to tune the electron-electron correlations in correlated oxides, the epitaxial strain induced variations in V-3d bandwidth, band center shift and band splitting at high symmetry points (${\Gamma}$, R) in SrVO$_3$ are investigated. The alterations in resistivity, carrier concentration, Hall coefficient and plasma frequency with applied strain are also elucidated. Our calculations revealed that under tensile strain, the lifting of the threefold degeneracy of 3d-t$_{2g}$ orbital and d-band narrowing reinforces a relatively less conducting state thus limiting the $\omega_P$ to lower frequencies. On the contrary, in case of compressive strain the d-band widening predominates leading to an increase in carrier concentration and decrease in resistivity enhancing the metallic state. As a result, $\omega_P$ is increased to higher frequencies which decreases the optical transparency window. Hence, our results and findings clearly demonstrate the interdependence between the optical and transport properties, and provides a detailed mechanism to tune the optoelectronic properties of SrVO$_3$ for its applications as a transparent conducting oxide.",2212.05449v1 2022-12-19,Optical Switching in Tb/Co-Multilayer Based Nanoscale Magnetic Tunnel Junctions,"Magnetic tunnel junctions (MTJs) are elementary units of magnetic memory devices. For high-speed and low-power data storage and processing applications, fast reversal by an ultrashort laser pulse is extremely important. We demonstrate optical switching of Tb/Comultilayer-based nanoscale MTJs by combining optical writing and electrical read-out methods. A 90 fs-long laser pulse switches the magnetization of the storage layer (SL). The change in magnetoresistance between the SL and a reference layer (RL) is probed electrically across the tunnel barrier. Single-shot switching is demonstrated by varying the cell diameter from 300 nm to 20 nm. The anisotropy, magnetostatic coupling, and switching probability exhibit cell-size dependence. By suitable association of laser fluence and magnetic field, successive commutation between high-resistance and low-resistance states is achieved. The switching dynamics in a continuous film is probed with the magneto-optical Kerr effect technique. Our experimental findings provide strong support for the growing interest in ultrafast spintronic devices.",2212.10361v1 2023-02-02,Controlling the Skyrmion Density and Size for Quantized Convolutional Neural Networks,"Skyrmion devices show energy efficient and high integration data storage and computing capabilities. Herein, we present the results of experimental and micromagnetic investigations of the creation and stability of magnetic skyrmions in the Ta/IrMn/CoFeB/MgO thin film system. We investigate the magnetic-field dependence of the skyrmion density and size using polar magneto optical Kerr effect MOKE microscopy supported by a micromagnetic study. The evolution of the topological charge with time under a magnetic field is investigated, and the transformation dynamics are explained. Furthermore, considering the voltage control of these skyrmion devices, we evaluate the dependence of the skyrmion size and density on the Dzyaloshinskii Moriya interaction and the magnetic anisotropy. We furthermore propose a skyrmion based synaptic device based on the results of the MOKE and micromagnetic investigations. We demonstrate the spin-orbit torque controlled discrete topological resistance states with high linearity and uniformity in the device. The discrete nature of the topological resistance makes it a good candidate to realize hardware implementation of weight quantization in a quantized neural network (QNN). The neural network is trained and tested on the CIFAR10 dataset, where the devices act as synapses to achieve a recognition accuracy of 87%, which is comparable to the result of ideal software-based methods.",2302.01390v1 2023-03-04,High pressure ferroelectric-like semi-metallic state in $Eu-$doped $BaTiO_3$,"We have conducted a detailed high-pressure (HP) investigation on $Eu-$doped $BaTiO_3$ using angle-resolved x-ray diffraction, Raman spectroscopy, dielectric permittivity and dc resistance measurements. The x-ray diffraction data analysis shows a pressure-induced structural phase transition from the ambient tetragonal to the mixed cubic and tetragonal phase above 1.4 GPa. The tetragonality of the sample due to the internal deformation of the $TiO_6$ octahedra caused by charge difference from Eu doping cannot be lifted upon by pressure. Softening, weakening, and disappearance of low-frequency Raman modes indicate ferroelectric tetragonal to the paraelectric cubic phase transition. But the pressure-induced increase in the intensity of [E(LO), A1(LO)] and the octahedral breathing modes indicate the local structural inhomogeneity remains in the crystal and is responsible for spontaneous polarization in the sample. Low-frequency electronic scattering response suggests the pressure-induced carrier delocalization, leading to a semi-metallic state in the system. Our HP dielectric constant and dc resistance data can be explained by the presence of pressure-induced localized clusters of microscopic ferroelectric ordering. Our results suggest HP phase coexistence leads to a ferroelectric-like semi-metallic state in $Eu-$doped $BaTiO_3$ under the extreme quantum limit.",2303.02329v2 2023-09-21,"High-Conductance, Ohmic-like HfZrO$_4$ Ferroelectric Memristor","The persistent and switchable polarization of ferroelectric materials based on HfO$_2$-based ferroelectric compounds, compatible with large-scale integration, are attractive synaptic elements for neuromorphic computing. To achieve a record current density of 0.01 A/cm$^2$ (at a read voltage of 80 mV) as well as ideal memristive behavior (linear current-voltage relation and analog resistive switching), devices based on an ultra-thin (2.7 nm thick), polycrystalline HfZrO$_4$ ferroelectric layer are fabricated by Atomic Layer Deposition. The use of a semiconducting oxide interlayer (WO$_{x<3}$) at one of the interfaces, induces an asymmetric energy profile upon ferroelectric polarization reversal and thus the long-term potentiation / depression (conductance increase / decrease) of interest. Moreover, it favors the stable retention of both the low and the high resistive states. Thanks to the low operating voltage (<3.5 V), programming requires less than 10${^-12}$ J for 20 ns long pulses. Remarkably, the memristors show no wake-up or fatigue effect.",2309.12070v1 2023-12-27,"Inkjet-Printed High-Yield, Reconfigurable, and Recyclable Memristors on Paper","Reconfigurable memristors featuring neural and synaptic functions hold great potential for neuromorphic circuits by simplifying system architecture, cutting power consumption, and boosting computational efficiency. Their additive manufacturing on sustainable substrates offers unique advantages for future electronics, including low environmental impact. Here, exploiting structure-property relationship of MoS2 nanoflake-based resistive layer, we present paper-based, inkjet-printed, reconfigurable memristors. With >90% yield from a 16x65 device array, our memristors demonstrate robust resistive switching, with $>10^5$ ON-OFF ratio and <0.5 V operation in non-volatile state. Through modulation of compliance current, the devices transition into volatile state, with only 50 pW switching power consumption, rivalling state-of-the-art metal oxide-based counterparts. We show device recyclability and stable, reconfigurable operation following disassembly, material collection and re-fabrication. We further demonstrate synaptic plasticity and neuronal leaky integrate-and-fire functionality, with disposable applications in smart packaging and simulated medical image diagnostics. Our work shows a sustainable pathway towards printable, high-yield, reconfigurable neuromorphic devices, with minimal environmental footprint.",2312.16501v1 2018-06-20,Linear-$T$ resistivity at high temperature,"The linear-$T$ resistivity is one of the characteristic and universal properties of strange metals. There have been many progress in understanding it from holographic perspective (gauge/gravity duality). In most holographic models, the linear-$T$ resistivity is explained by the property of the infrared geometry and valid at low temperature limit. On the other hand, experimentally, the linear-$T$ resistivity is observed in a large range of temperatures, up to room temperature. By using holographic models related to the Gubser-Rocha model, we investigate how much the linear-$T$ resistivity is robust at higher temperature above the superconducting phase transition temperature. We find that strong momentum relaxation plays an important role to have a robust linear-$T$ resistivity up to high temperature.",1806.07739v2 2018-07-18,Multi-band effects in in-plane resistivity anisotropy of strain-detwinned disordered Ba(Fe$_{1-x}$Ru$_{x}$)$_{2}$As$_{2}$,"In-plane resistivity anisotropy was measured in strain-detwinned as-grown and partially annealed samples of isovalently-substituted $\mathrm{Ba(Fe_{1-x}Ru_{x})_{2}As_{2}}$ ($0 hcp phase transition.",1007.3423v1 2010-08-11,Contact resistivity and current flow path at metal/graphene contact,"The contact properties between metal and graphene were examined. The electrical measurement on a multiprobe device with different contact areas revealed that the current flow preferentially entered graphene at the edge of the contact metal. The analysis using the cross-bridge Kelvin structure (CBK) suggested that a transition from the edge conduction to area conduction occurred for a contact length shorter than the transfer length of ~1 micron. The contact resistivity for Ni was measured as ~5*10-6 Ohmcm2 using the CBK. A simple calculation suggests that a contact resistivity less than 10-9 Ohmcm2 is required for miniaturized graphene field effect transistors.",1008.1826v1 2010-12-05,Snake States in Graphene p-n Junctions,"We investigate transport in locally-gated graphene devices, where carriers are injected and collected along, rather than across, the gate edge. Tuning densities into the p-n regime significantly reduces resistance along the p-n interface, while resistance across the interface increases. This provides an experimental signature of snake states, which zig-zag along the p-n interface and remain stable as applied perpendicular magnetic field approaches zero. Snake states appear as a peak in transverse resistance measured along the p-n interface. The generic role of snake states disordered graphene is also discussed.",1012.0959v2 2011-08-18,Non-volatile Complementary Resistive Switch-based Content Addressable Memory,"This paper presents a novel resistive-only Binary and Ternary Content Addressable Memory (B/TCAM) cell that consists of two Complementary Resistive Switches (CRSs). The operation of such a cell relies on a logic$\rightarrow$ON state transition that enables this novel CRS application.",1108.3716v2 2012-11-16,Universal scaling of resistivity in bilayer graphene,"We report the temperature dependent electrical transport properties of gated bilayer graphene devices. We see a clear evidence of insulating behavior due to electron-hole charge puddles. The electrical resistivity increases while the mobility decreases with decreasing temperature, a characteristic due to carrier inhomogeneity in graphene. The theoretical fittings using an empirical formula of single electron tunneling indicate that electrical resistivity follows a universal curve with a scaling parameter. The scaling parameter is determined to be a measure of the fluctuations in the electron-hole puddle distribution.",1211.3807v1 2013-04-15,Many Topological Insulators Fail the Surface Conduction Test,"In this report, we scrutinize the thickness dependent resistivity data from the recent literature on electrical transport measurements in topological insulators. A linear increase in resistivity with increase in thickness is expected in the case of these materials since they have an insulating bulk and conducting surface. However, such a trend is not seen in the resistivity versus thickness data for all the cases examined, except for some samples, where it holds for a narrow range of thickness.",1304.4037v2 2014-04-14,Giant generic topological Hall resistivity of MnSi under pressure,"We report detailed low temperature magnetotransport and magnetization measurements in MnSi under pressures up to $\sim12\,{\rm kbar}$. Tracking the role of sample quality, pressure transmitter, and field and temperature history allows us to link the emergence of a giant topological Hall resistivity $\sim50\,{\rm n\Omega cm}$ to the skyrmion lattice phase at ambient pressure. We show that the remarkably large size of the topological Hall resistivity in the zero-temperature limit must be generic. We discuss various mechanisms which can lead to the much smaller signal at elevated temperatures observed at ambient pressure.",1404.3734v1 2015-01-27,The Vacancy Effect on Thermal Interface Resistance between Aluminum and Silicon by Molecular Dynamics,"Thermal transport across interfaces is an important issue for microelectronics, photonics, and thermoelectric devices and has been studied both experimentally and theoretically in the past. In this paper, thermal interface resistance (1/G) between aluminum and silicon with nanoscale vacancies was calculated using non-equilibrium molecular dynamics (NEMD). Both phonon-phonon coupling and electron-phonon coupling are considered in calculations. The results showed that thermal interface resistance increased largely due to vacancies. The effect of both the size and the type of vacancies is studied and compared. And an obvious difference is found for structures with different type/size vacancies.",1501.06666v1 2015-03-12,"Comment on ""Correlation between Bulk Thermodynamic Measurements and the Low-Temperature-Resistance Plateau in SmB6""","Low-temperature-resistivity plateau observed in $\rm SmB_6$ single crystal,which is due to surface, not bulk, conduction has been confirmed from electrical transport measurements. Recently, the correlation between bulk thermodynamic measurements and the low-temperature-resistance plateau in $\rm SmB_6$ have been investigated and a change in Sm valence at the surface has been obtained from x-ray absorption spectroscopy and x-ray magnetic circular dichroism. Here we show that the statement of the report are not supported by the results from x-ray absorption spectroscopy and x-ray magnetic circular dichroism.",1503.03901v1 2015-05-14,On the vanishing resistivity limit and the magnetic boundary-layers for one-dimensional compressible magnetohydrodynamics,"We consider an initial-boundary value problem for the one-dimensional equations of compressible isentropic viscous and non-resistive magnetohydrodynamic flows. The global well-posedness of strong solutions with general large data is established. Moreover, the vanishing resistivity limit is justified and the thickness of magnetic boundary layers is analyzed. The proofs of these results are based on a full use of the so-called ""effective viscous flux"", the material derivative and the structure of the equations.",1505.03596v1 2017-02-06,A thermodynamic theory of filamentary resistive switching,"We present a phenomenological theory of filamentary resistive random access memory (RRAM) describing the commonly observed features of their current-voltage characteristics. Our approach follows the approach of thermodynamic theory developed earlier for chalcogenide memory and threshold switches and largely independent of their microscopic details. It explains, without adjustable parameters, such features as the domains of filament formation and switching, voltage independent current in SET and current independent voltage in RESET regimes, the relation between the set and reset voltages, filament resistance independent of its length, etc. Furthermore, it expresses the observed features through the material and circuitry parameters thus paving a way to device improvements.",1702.01480v1 2017-10-02,Electrical resistivity across the tricriticality in itinerant ferromagnet,"We investigate the discontinuous ferromagnetic phase diagram near tricritical point in UCo 1-x Ru x Al compounds by electrical resistivity measurements. Separation of phases in UCo 0.995 Ru 0.005 Al at ambient pressure and in UCo 0.990 Ru 0.010 Al at pressure of 0.2 GPa and disappearance of ferromagnetism at 0.4 GPa is confirmed. The exponent of temperature dependence of electrical resistivity implies change from Fermi liquid behavior to non-Fermi liquid at 0.2 GPa and reaches minimum at 0.4 GPa. Our results are compared to results obtained on the pure UCoAl and explanation for different exponents is given.",1710.00860v1 2017-10-04,Towards Replacing Resistance Thermometry with Photonic Thermometry,"Resistance thermometry provides a time-tested method for taking temperature measurements that has been painstakingly developed over the last century. However, fundamental limits to resistance-based approaches along with a desire to reduce the cost of sensor ownership and increase sensor stability has produced considerable interest in developing photonic temperature sensors. Here we demonstrate that silicon photonic crystal cavity-based thermometers can measure temperature with uncertainities of 175 mK (k = 1), where uncertainties are dominated by ageing effects originating from the hysteresis in the device packaging materials. Our results, a 4-fold improvement over recent developments, clearly demonstate the rapid progress of silicon photonic sensors in replacing legacy devices.",1710.01704v1 2018-09-28,Thermal resistance of GaN/AlN graded interfaces,"Compositionally graded interfaces in power electronic devices eliminate dislocations, but they can also decrease thermal conduction, leading to overheating. We quantify the thermal resistances of GaN/AlN graded interfaces of varying thickness using ab initio Green's functions, and compare them with the abrupt interface case. A non-trivial power dependence of the thermal resistance versus interface thickness emerges from the interplay of alloy and mismatch scattering mechanisms. We show that the overall behavior of such graded interfaces is very similar to that of a thin-film of an effective alloy in the length scales relevant to real interfaces.",1809.11046v2 2017-03-08,Resistive Switching in Memristive Electrochemical Metallization Devices,"We report on resistive switching of memristive electrochemical metallization devices using 3D kinetic Monte Carlo simulations describing the transport of ions through a solid state electrolyte of an Ag/TiO$_{\text{x}}$/Pt thin layer system. The ion transport model is consistently coupled with solvers for the electric field and thermal diffusion. We show that the model is able to describe not only the formation of conducting filaments but also its dissolution. Furthermore, we calculate realistic current-voltage characteristics and resistive switching kinetics. Finally, we discuss in detail the influence of both the electric field and the local heat on the switching processes of the device.",1703.02946v2 2012-01-31,"Magnetoresistance, noise properties and the Koshino-Taylor effect in the quasi-1D oxide KRu_4O_8","The low temperature electronic and galvanomagnetic transport properties of the low dimensional oxide KRu_4O_8 are experimentally considered. A quadratic temperature variation of the resistivity is observed to be proportional to the residual resistivity. It shows the role of inelastic electron scattering against impurities, i.e. a large Koshino-Taylor effect, rather than a consequence of strong electronic correlations. In the same temperature range, the Kohler rule is not fulfilled. The resistance noise increases also sharply, possibly due to a strong coupling of carriers with lattice fluctuations in this low dimensional compound.",1201.6474v1 2022-07-12,A Simple and Precise Way to Determine Electrical Resistivity of Isotropic Conductors: Simplifying the Four-Probe Method,"COMSOL Multiphysics software is used to describe the behavior of the electrical resistivity of several samples with rectangular shape typically used in the Montgomery method. The simulation data obtained using four isotropic conductors allowed us to understand in detail the behavior of the electric potential and electric field of the samples. The results provide an analytical method which can substitute the four-probe method with much more simplicity and precision.",2207.05863v1 2022-11-08,Role of the annealing parameters on the resistance of indium tin oxide nanocrystalline films,"The optical and electrical properties of films made of nanoparticles of indium tin oxide (ITO) are widely studied because of the significance of this material for transparent electrodes, smart windows, and nonlinear optics components. In this work, a systematic study of the resistance in ITO nanocrystalline films, as a function of post-fabrication parameters, such as the temperature and time of annealing, has been performed. A tunability of the resistance with the annealing parameters, in a range of three orders of magnitude, has been demonstrated.",2211.04144v2 2023-11-16,Measuring the Kapitza Resistance between a Passivated Semiconductor and Liquid Helium,"In this paper, we describe an experimental investigation into the effect of passivation layer thickness on heat dissipation between a quartz substrate and liquid helium. We have observed that by depositing SiN from 0 to 240 nm, the Kapitza resistance increases by 0.0365 m^2.K/W per nanometer more than for an unpassivated semiconductor. We hypothesize that this increase in Kapitza resistance represents an additional barrier to the cooling of semiconductor devices in liquid helium.",2312.03713v1 2021-07-26,Laser-equipped gas reaction chamber for probing environmentally sensitive materials at near atomic scale,"Numerous metallurgical and materials science applications depend on quantitative atomic-scale characterizations of environmentally-sensitive materials and their transient states. Studying the effect upon materials subjected to thermochemical treatments in specific gaseous atmospheres is of central importance for specifically studying a material's resistance to certain oxidative or hydrogen environments. It is also important for investigating catalytic materials, direct reduction of an oxide, particular surface science reactions or nanoparticle fabrication routes. This manuscript realizes such experiments upon a thermochemical reaction chamber called the Reacthub and allows for transferring treated materials under cryogenic & ultrahigh vacuum workflow conditions for characterisation by either atom probe or scanning Xe+/electron microscopies. Two examples are discussed in the present study. One protocol was in the deuterium gas charging (25 kPa D2 at 200 {\deg}C) of a high-manganese twinning-induced-plasticity steel and characterization of the ingress and trapping of hydrogen at various features (grain boundaries in particular) in efforts to relate this to the steel's hydrogen embrittlement susceptibility. Deuterium was successfully detected after gas charging but most contrast originated from the complex ion FeOD+ signal and the feature may be an artefact. The second example considered the direct deuterium reduction (5 kPa D2 at 700 {\deg}C) of a single crystal wuestite sample, demonstrating that under a standard thermochemical treatment causes rapid reduction upon the nanoscale. Further studies are required for complete confidence about these phenomena, but these experiments successfully demonstrate that how an ex-situ thermochemical treatment can be realised that captures environmentally-sensitive transient states that can be analysed by atomic-scale by atom probe microscope.",2107.11987v2 2023-03-19,2D MXene Electrochemical Transistors,"In the past two decades another transistor based on conducting polymers, called the organic electrochemical transistor (ECT) was shown and largely studied. The main difference between organic ECTs and FETs is the mode and extent of channel doping: while in FETs the channel only has surface doping through dipoles, the mixed ionic-electronic conductivity of the channel material in Organic ECTs enables bulk electrochemical doping. As a result, the organic ECT maximizes conductance modulation at the expense of speed. Until now ECTs have been based on conducting polymers, but here we show that MXenes, a class of 2D materials beyond graphene, have mixed ionic-electronic properties that enable the realization of electrochemical transistors (ECTs). We show that the formulas for organic ECTs can be applied to these 2D ECTs and used to extract parameters like mobility. These MXene ECTs have high transconductance values but low on-off ratios. We further show that conductance switching data measured using ECT, in combination with other in-situ ex-situ electrochemical measurements, is a powerful tool for correlating the change in conductance to that of redox state: to our knowledge, this is the first report of this important correlation for MXene films. Many future possibilities exist for MXenes ECTs, and we think other 2D materials with bandgaps can also form ECTs with single or heterostructured 2D materials. 2D ECTs can draw great inspiration and theoretical tools from the field of organic ECTs and have the potential to considerably extend the capabilities of transistors beyond that of conducting polymer ECTs, with added properties such as extreme heat resistance, tolerance for solvents, and higher conductivity for both electrons and ions than conducting polymers.",2303.10768v2 2016-02-10,Electronic Evidence of Temperature-Induced Lifshitz Transition and Topological Nature in ZrTe5,"The topological materials have attracted much attention recently. While three-dimensional topological insulators are becoming abundant, two-dimensional topological insulators remain rare, particularly in natural materials. ZrTe5 has host a long-standing puzzle on its anomalous transport properties; its underlying origin remains elusive. Lately, ZrTe5 has ignited renewed interest because it is predicted that single-layer ZrTe5 is a two-dimensional topological insulator and there is possibly a topological phase transition in bulk ZrTe5. However, the topological nature of ZrTe5 is under debate as some experiments point to its being a three-dimensional or quasi-two-dimensional Dirac semimetal. Here we report high-resolution laser-based angle-resolved photoemission measurements on ZrTe5. The electronic property of ZrTe5 is dominated by two branches of nearly-linear-dispersion bands at the Brillouin zone center. These two bands are separated by an energy gap that decreases with decreasing temperature but persists down to the lowest temperature we measured (~2 K). The overall electronic structure exhibits a dramatic temperature dependence; it evolves from a p-type semimetal with a hole-like Fermi pocket at high temperature, to a semiconductor around ~135 K where its resistivity exhibits a peak, to an n-type semimetal with an electron-like Fermi pocket at low temperature. These results indicate a clear electronic evidence of the temperature-induced Lifshitz transition in ZrTe5. They provide a natural understanding on the underlying origin of the resistivity anomaly at ~135 K and its associated reversal of the charge carrier type. Our observations also provide key information on deciphering the topological nature of ZrTe5 and possible temperature-induced topological phase transition.",1602.03576v1 2010-11-11,Nonlinear Insulator in Complex Oxides,"The insulating state is one of the most basic electronic phases in condensed matter. This state is characterised by an energy gap for electronic excitations that makes an insulator electrically inert at low energy. However, for complex oxides, the very concept of an insulator must be re-examined. Complex oxides behave differently from conventional insulators such as SiO2, on which the entire semiconductor industry is based, because of the presence of multiple defect levels within their band gap. As the semiconductor industry is moving to such oxides for high-dielectric (high-k) materials, we need to truly understand the insulating properties of these oxides under various electric field excitations. Here we report a new class of material called nonlinear insulators that exhibits a reversible electric-field-induced metal-insulator transition. We demonstrate this behaviour for an insulating LaAlO3 thin film in a metal/LaAlO3/Nb-SrTiO3 heterostructure. Reproducible transitions were observed between a low-resistance metallic state and a high-resistance non-metallic state when applying suitable voltages. Our experimental results exclude the possibility that diffusion of the metal electrodes or oxygen vacancies into the LaAlO3 layer is occurring. Instead, the phenomenon is attributed to the formation of a quasi-conduction band (QCB) in the defect states of LaAlO3 that forms a continuum state with the conduction band of the Nb-SrTiO3. Once this continuum (metallic) state is formed, the state remains stable even when the voltage bias is turned off. An opposing voltage is required to deplete the charges from the defect states. Our ability to manipulate and control these defect states and, thus, the nonlinear insulating properties of complex oxides will open up a new path to develop novel devices.",1011.2629v1 2022-08-31,CeFe$_2$Al$_{10}$: a Correlated Metal with a Fermi Surface Exhibiting Nonmetallic Conduction,"Metals can be defined as materials with a Fermi surface or as materials exhibiting metallic conduction (i.e., $\mathrm{d} \rho / \mathrm{d}T > 0$). Usually, these definitions both hold at low temperatures, such as liquid-helium temperatures, as the Fermi energy is sufficiently larger than the thermal energy. However, they may not both hold in correlated electron systems where the Fermi energy is reduced by renormalization. In this paper, we demonstrate that although the resistivity of CeFe$_2$Al$_{10}$ increases with decreasing temperature below $\sim20$ K, CeFe$_2$Al$_{10}$ is a metal with a Fermi surface. This assertion is based on the observation of Shubnikov--de Haas oscillations and a Hall resistivity that changes sign with the magnetic field, which requires the coexistence of electron and hole carriers. Our analysis of Shubnikov--de Haas and magnetotransport data indicates that the Fermi energies are as small as $\sim$30 K and that, despite the increasing carrier mobility with decreasing temperature as in conventional metals, the loss of thermally excited carriers leads to nonmetallic conduction ($\mathrm{d} \rho / \mathrm{d}T < 0$) below $\sim20$ K. Furthermore, we investigate how this anomalous metal transforms to a more conventional metal with metallic conduction by the application of high pressure and a high magnetic field. This study illustrates the subtle distinction between semimetals and semiconductors in correlated electron systems. This distinction is relevant to investigations of correlated topological insulators and semimetals.",2208.14630v4 2011-08-08,KEK effort for high field magnets,"KEK has emphasized efforts to develop the RHQNb3Al superconductor and a sub-scale magnet reaching 13 T towards the HL-LHC upgrade in last years. In addition, relevant R&D regarding radiation resistance has been carried out. For higher field magnets beyond 15 T, HTS in combination with A15 superconductors should be one of baseline materials. However, all these superconductors are very sensitive to stress and strain and thorough understanding of behaviour is truly desired for realization of high field magnets. KEK has launched a new research subject on stress/strain sensitivity of HTS and A15 superconductors in collaboration with the neutron diffraction facility at J-PARC and High Field Laboratory in Tohoku University. Present activity for high field magnets at KEK is reported.",1108.1626v1 2013-10-29,Fabrication of single-walled carbon nanotube/Si heterojunction solar cell with high photovoltaic conversion efficiency and stability,"The photovoltaic properties of carbon nanotube/Si heterojunction solar cells were investigated using network films of high quality single-walled carbon nanotubes (SWNTs) grown by atmospheric-pressure floating-catalyst chemical vapor deposition. Because of the optimization of the device window size and the utilization of SWNT thin films with both low resistivity and high transparency, a high photovoltaic conversion efficiency of greater than 12% was achieved for SWNTs/Si heterojunction solar cells without any post processing, such as carrier doping treatment. In addition, the high stability and reproducibility of the photovoltaic performance of these devices in air was demonstrated.",1310.7783v2 2021-02-15,Fermi-surface reconstruction at the metamagnetic high-field transition in uranium mononitride,"We report on the electronic and thermodynamic properties of the antiferromagnetic metal uranium mononitride with a N\'eel temperature $T_N\approx 53\,$K. The fabrication of microstructures from single crystals enables us to study the low-temperature metamagnetic transition at approximately $58\,$T by high-precision magnetotransport, Hall-effect, and magnetic-torque measurements. We confirm the evolution of the high-field transition from a broad and complex behavior to a sharp first-order-like step, associated with a spin flop at low temperature. In the high-field state, the magnetic contribution to the temperature dependence of the resistivity is suppressed completely. It evolves into an almost quadratic dependence at low temperatures indicative of a metallic character. Our detailed investigation of the Hall effect provides evidence for a prominent Fermi-surface reconstruction as the system is pushed into the high-field state.",2102.07512v2 2020-06-17,Electrical transport measurements for superconducting sulfur hydrides using boron-doped diamond electrodes on beveled diamond anvil,"A diamond anvil cell (DAC) which can generate extremely high pressure of multi-megabar is promising tool to develop a further physics such a high-transition temperature superconductivity. However, electrical transport measurements, which is one of the most important properties of such functional materials, using the DAC is quite difficult because the sample space is very small and a deformation of electrodes under extreme condition. In this study, we fabricated a boron-doped diamond micro-electrode and an undoped diamond insulation on a beveled culet surface of the diamond anvil. By using the developed DAC, we demonstrated the electrical transport measurements for sulfur hydride H$_2$S which known as a pressure-induced high-transition temperature superconducting H$_3$S at high pressure. The measurements were successfully conducted under high pressure up to 192 GPa, and then a multi-step superconducting transition composed from pure sulfur and some kinds of surfer hydrides, which is possible HS$_2$, was observed with zero resistance.",2006.09671v1 2023-10-02,Thermoelectric properties of high-entropy wolframite oxide: (CoCuNiFeZn)$_{1-x}$Ga$_x$WO$_4$,"In this report, the synthesis of high-entropy wolframite oxide (CoCuNiFeZn)$_{1-x}$Ga$_x$WO$_4$ through standard solid-state route followed by spark plasma sintering (SPS) and their structural, microstructural, and thermoelectric properties are investigated. X-ray diffraction pattern followed by pattern matching refinement shows monoclinic structure with volume of the unit cell decreasing with increasing Ga content. The optical band gap for these oxides shows a cocktail effect in high entropy configuration. The Seebeck coefficient indicates electrons as dominating charge carriers with a non-degenerate behavior. The electrical resistivity decreases with increasing temperature depicting a semiconducting nature. Thermal conductivity in high-entropy samples ($\kappa\sim$2.1 W/mK @ 300\,K) is significantly lower as compared to MgWO$_4$ ($\kappa\sim$11.5 W/mK @ 300\,K), which can be explained by the strong phonon scattering due to large lattice disorder in high entropy configuration. The thermoelectric figure of merit zT increases with Ga doping via modifying all three thermoelectric parameters positively.",2310.00930v1 1999-03-01,Anisotropic resistivity of the antiferromagnetic insulator Bi_2Sr_2ErCu_2O_8,"Anisotropic resistivities of Bi_2Sr_2Ca_{1-x}Er_xCu_2O_8 single crystals were measured and analyzed from 4.2 to 500 K with special interest in the parent antiferromagnetic insulator of x=1.0. Although the resistivity is semiconducting along both the in- and out-of-plane directions, the temperature dependence is found to be significantly different. As a result, the resistivity ratio for x=1.0 takes a broad maximum near room temperature. The electric conduction in parent antiferromagnetic insulators is different from other semiconductors, and is as unconventional as that in high-temperature superconductors.",9903023v2 2002-11-18,Transverse voltages and reciprocity theorem in magnetic fields for high T_c superconductors,"We have tested four-point methods of the Hall effect measurement on BiSrCaCuO (2223) polycrystal and also the validity of the magnetic field form of the reciprocity theorem. We found that different types of determination of the Hall resistance using various combination of measured resistances provide different value of it. We have separated two parts of the resistance combinations, which are even and odd in magnetic field, respectively. The odd part, which is equivalent to the Hall effect, is equal for all formulae used. The even part of transverse resistance varies in different formulae. The magnetic field form of the reciprocity theorem is not valid. Models for explanation of this violation are also discussed.",0211370v1 2003-06-03,Anomalous Flux Flow Resistivity in Two Gap Superconductor MgB_2,"The flux flow resistivity associated with purely viscous motion of vortices in high-quality MgB_2 was measured by microwave surface impedance. Flux flow resistivity exhibits unusual field dependence with strong enhancement at low field, which is markedly different to conventional s-wave superconductors. A crossover field which separates two distinct flux flow regimes having different flux flow resistivity slopes was clearly observed in H//ab-plane. The unusual H-dependence indicates that two very differently sized superconducting gaps in MgB_2 manifest in the vortex dynamics and almost equally contribute to energy dissipation. The carrier scattering rate in two different bands is also discussed with the present results, compared to heat capacity and thermal conductivity results.",0306057v1 2005-09-30,Valence fluctuation mediated superconductivity in CeCu2Si2,"It has been proposed that there are two types of superconductivity in CeCu2Si2, mediated by spin fluctuations at ambient pressure, and by critical valence fluctuations around a charge instability at a pressure P_v \simeq 4.5 GPa. We present in detail some of the unusual features of this novel type of superconducting state, including the coexistence of superconductivity and huge residual resistivity of the order of the Ioffe-Regel limit, large and pressure dependent resistive transition widths in a single crystal measured under hydrostatic conditions, asymmetric pressure dependence of the specific heat jump shape, unrelated to the resistivity width, and negative temperature dependence of the normal state resistivity below 10 K at very high pressure.",0509787v1 2007-06-05,Hall magnetoresistivity response under Microwave excitation revisited,"We theoretically analyzed the microwave-induced modification of the Hall magnetoresistivity in high mobility two-dimensional electron systems. These systems present diagonal magnetoresistivity oscillations and zero-resistance states when are subjected to microwave radiation. The most surprising modification of the Hall magnetoresistivity is a periodic reduction which correlates with a periodic increase in the diagonal resistivity. We present a model that explains the experimental results considering that radiation affects directly only the diagonal resistivity and the observed Hall resistivity changes are coming from the tensor relationship between both of them.",0706.0588v1 2009-06-22,Temperature dependent electrical resistivity of a single strand of ferromagnetic single crystalline nanowire,"We have measured the electrical resistivity of a single strand of a ferromagnetic Ni nanowire of diameter 55 nm using a 4-probe method in the temperature range 3 K-300 K. The wire used is chemically pure and is a high quality oriented single crystalline sample in which the temperature independent residual resistivity is determined predominantly by surface scattering. Precise evaluation of the temperature dependent resistivity ($\rho$) allowed us to identify quantitatively the electron-phonon contribution (characterized by a Debye temperature $\theta_R$) as well as the spin-wave contribution which is significantly suppressed upon size reduction.",0906.3903v1 2010-07-01,"First tests of ""bulk"" MICROMEGAS with resistive cathode mesh","We present the first results from tests of a MICROMEGAS detector manufactured using the so-called ""bulk"" technology and having a resistive cathode mesh instead of the conventional metallic one. This detector operates as usual MICROMEGAS, but in the case of sparks, which may appear at high gas gains, the resistive mesh reduces their current and makes the sparks harmless. This approach could be complementary to the ongoing efforts of various groups to develop spark-protected MICROMEGAS with resistive anode planes.",1007.0211v1 2010-07-08,Microwave zero-resistance states in a bilayer electron system,"Magnetotransport measurements on a high-mobility electron bilayer system formed in a wide GaAs quantum well reveal vanishing dissipative resistance under continuous microwave irradiation. Profound zero-resistance states (ZRS) appear even in the presence of additional intersubband scattering of electrons. We study the dependence of photoresistance on frequency, microwave power. and temperature. Experimental results are compared with a theory demonstrating that the conditions for absolute negative resistivity correlate with the appearance of ZRS.",1007.1393v1 2011-05-17,Microwave-induced Hall resistance in bilayer electron systems,"The influence of microwave irradiation on dissipative and Hall resistance in high-quality bilayer electron systems is investigated experimentally. We observe a deviation from odd symmetry under magnetic field reversal in the microwave-induced Hall resistance $\Delta R_{xy}$ whereas the dissipative resistance $\Delta R_{xx}$ obeys even symmetry. Studies of $\Delta R_{xy}$ as a function of the microwave electric field and polarization exhibit a strong and non-trivial power and polarization dependence. The obtained results are discussed in connection to existing theoretical models of microwave-induced photoconductivity.",1105.3362v1 2011-12-02,Mooij Rule and Weak Localization,"It has been shown that the observed correlation between the resistivity $\rho$ of high-resistive metallic alloys and the sign of the temperature derivative $d\rho/dT$ can be explained by taking into account the weak localization. This correlation is known as Mooij rule: the derivative $d\rho/dT$ is negative for alloys with resistivity in the range of $300\div150\,\mu\Omega\cdot$cm, which corresponds to the electron mean free path about the interatomic distance; however, this derivative is positive for alloys with lower resistivity.",1112.0429v1 2015-03-16,"High pressure investigation of superconducting signatures in CeCu$_{2}$Si$_{2}$ : ac- magnetic susceptibility and heat capacity, resistivity and thermopower","Taking advantage of a novel multiprobe setup we have measured, on a unique sample, the ac-magnetic susceptibility, the resistivity, the ac-specific heat and the thermopower of the superconductor heavy fermion CeCu$_{2}$Si$_{2}$ under pressure up to 5.1 GPa. At the superconducting transition temperature $T_c$, the Meissner signal corresponds to that expected for the sample volume and coincides with the specific heat jump and the resistive transition completion temperatures. Differing from previous observations, here the susceptibility measurements did not reveal any anomaly in the vicinity of the resistive transition onset.",1503.04861v2 2024-05-14,Experimental Demonstration of Turbulence-resistant Lidar via Quantum Entanglement,"We report a proof-of-principle experimental demonstration of a turbulence-resistant quantum Lidar system. As a key technology for sensing and ranging, Lidar has drawn considerable attention for a study from quantum perspective, in search of proven advantages complementary to the capabilities of conventional Lidar technologies. Environmental factors such as strong atmospheric turbulence can have detrimental effects on the performance of these systems. We demonstrate the possibility of turbulence-resistant operation of a quantum Lidar system via two-photon interference of entangled photon pairs. Additionally, the reported quantum Lidar also demonstrates the expected noise resistance. This study suggests a potential high precision timing-positioning technology operable under turbulence and noise.",2405.08916v1 2020-11-26,Systematic study of nonmagnetic resistance changes due to electrical pulsing in single metal layers and metal/antiferromagnet bilayers,"Intense current pulses are often required to operate microelectronic and spintronic devices. Notably, strong current pulses have been shown to induce magnetoresistance changes attributed to domain reorientation in antiferromagnet/heavy metal bilayers and non-centrosymmetric antiferromagnets. In such cases, nonmagnetic resistivity changes may dominate over signatures of antiferromagnetic switching. We report systematic measurements of the current-induced changes of the transverse and longitudinal resistance of Pt and Pt/NiO layers deposited on insulating substrates, namely Si/SiO$_2$, Si/Si$_3$N$_4$, and Al$_2$O$_3$. We identify the range of pulse amplitude and length that can be used without affecting the resistance and show that it increases with the device size and thermal diffusivity of the substrate. No significant difference is observed in the resistive response of Pt and NiO/Pt devices, thus precluding evidence on the switching of antiferromagnetic domains in NiO. The variation of the transverse resistance is associated to a thermally-activated process in Pt that decays following a double exponential law with characteristic timescales of a few minutes to hours. We use a Wheatstone bridge model to discriminate between positive and negative resistance changes, highlighting competing annealing and electromigration effects. Depending on the training of the devices, the transverse resistance can either increase or decrease between current pulses. Further, we elucidate the origin of the nonmonotonic resistance baseline, which we attribute to training effects combined with the asymmetric distribution of the current. These results provide insight into the origin of current-induced resistance changes in metal layers and a guide to minimize nonmagnetic artifacts in switching experiments of antiferromagnets.",2011.13413v1 2013-04-17,Universal density scaling of disorder-limited low-temperature conductivity in high-mobility two-dimensional systems,"We theoretically consider the carrier density dependence of low-temperature electrical conductivity in high-quality and low-disorder two-dimensional (2D) `metallic' electronic systems such as 2D GaAs electron or hole quantum wells or gated graphene. Taking into account resistive scattering by Coulomb disorder arising from quenched random charged impurities in the environment, we show that the 2D conductivity \sigma(n) varies as \sigma ~ n^{\beta(n)} as a function of the 2D carrier density n where the exponent \beta(n) is a smooth, but non-monotonic, function of density with possible nontrivial extrema. In particular, the density scaling exponent \beta(n) depends qualitatively on whether the Coulomb disorder arises primarily from remote or background charged impurities or short-range disorder, and can, in principle, be used to characterize the nature of the dominant background disorder. A specific important prediction of the theory is that for resistive scattering by remote charged impurities, the exponent \beta can reach a value as large as 2.7 for k_F d ~ 1, where k_F ~\sqrt{n} is the 2D Fermi wave vector and d is the separation of the remote impurities from the 2D layer. Such an exponent \beta (>5/2) is surprising because unscreened Coulomb scattering by remote impurities gives a limiting theoretical scaling exponent of \beta = 5/2, and naively one would expect \beta(n) \le 5/2 for all densities since unscreened Coulomb scattering should nominally be the situation bounding the resistive scattering from above. We find numerically and show theoretically that the maximum value of \alpha (\beta), the mobility (conductivity) exponent, for 2D semiconductor quantum wells is around 1.7 (2.7) for all values of d (and for both electrons and holes) with the maximum \alpha occurring around k_F d ~ 1. We discuss experimental scenarios for the verification of our theory.",1304.4668v1 2014-03-16,Comparison of Sn-doped and nonstoichiometric vertical-Bridgman-grown crystals of the topological insulator Bi2Te2Se,"A comparative study of the properties of topological insulator Bi2Te2Se (BTS) crystals grown by the vertical Bridgeman method is described. Two defect mechanisms that create acceptor impurities to compensate for the native n-type carriers are compared: Bi excess, and light Sn doping. Both methods yield low carrier concentrations and an n-p crossover over the length of the grown crystal boules, but lower carrier concentrations and higher resistivities are obtained for the Sn-doped crystals, which reach carrier concentrations as low as 8 x 1014 cm-3. Further, the temperature dependent resistivities for the Sn-doped crystals display strongly activated behavior at high temperatures, with a characteristic energy of half the bulk band gap. The (001) cleaved Sn-doped BTS crystals display high quality Shubnikov de Haas (SdH) quantum oscillations due to the topological surface state electrons. Angle resolved photoelectron spectroscopy (ARPES) characterization shows that the Fermi energy (EF) for the Sn-doped crystals falls cleanly in the surface states with no interference from the bulk bands, that the Dirac point for the surface states lies approximately 60 meV below the top of the bulk valence band maximum, and allows for a determination of the bulk and surface state carrier concentrations as a function of Energy near EF. Electronic structure calculations that compare Bi excess and Sn dopants in BTS demonstrate that Sn acts as a special impurity, with a localized impurity band that acts as a charge buffer occurring inside the bulk band gap. We propose that the special resonant level character of Sn in BTS gives rise to the exceptionally low carrier concentrations and activated resistivities observed.",1403.3870v1 2015-02-13,Epitaxial graphene on SiC: Modification of structural and electron transport properties by substrate pretreatment,"The electrical transport properties of epitaxial graphene layers are correlated with the SiC surface morphology. In this study we show by atomic force microscopy and Raman measurements that the surface morphology and the structure of the epitaxial graphene layers change significantly when different pretreatment procedures are applied to nearly on-axis 6H-SiC(0001) substrates. It turns out that the often used hydrogen etching of the substrate is responsible for undesirable high macro steps evolving during graphene growth. A more advantageous type of sub-nanometer stepped graphene layers is obtained with a new method: a high-temperature conditioning of the SiC surface in argon atmosphere. The results can be explained by the observed graphene buffer layer domains after the conditioning process which suppress giant step bunching and graphene step flow growth. The superior electronic quality is demonstrated by a less extrinsic resistance anisotropy obtained in nano-probe transport experiments and by the excellent quantization of the Hall resistance in low-temperature magneto-transport measurements. The quantum Hall resistance agrees with the nominal value (half of the von Klitzing constant) within a standard deviation of 4.5*10(-9) which qualifies this method for the fabrication of electrical quantum standards.",1502.03927v3 2020-07-09,"Growth, Properties, and Applications of Pulsed Laser Deposited Nanolaminate Ti3AlC2 Thin Films","Recently, nanolaminated ternary carbides have attracted immense interest due to the concomitant presence of both ceramic and metallic properties. Here, we grow nanolaminate Ti3AlC2 thin films by pulsed laser deposition on c-axis-oriented sapphire substrates and, surprisingly, the films are found to be highly oriented along the (103) axis normal to the film plane, rather than the (000l) orientation. Multiple characterization techniques are employed to explore the structural and chemical quality of these films, the electrical and optical properties, and the device functionalities. The 80-nm thick Ti3AlC2 film is highly conducting at room temperature (resistivity of 50 micro ohm-cm), and a very-low-temperature coefficient of resistivity. The ultrathin (2 nm) Ti3AlC2 film has fairly good optical transparency and high conductivity at room temperature (sheet resistance of 735 ohm). Scanning tunneling microscopy reveals the metallic characteristics (with finite density of states at the Fermi level) at room temperature. The metal-semiconductor junction of the p-type Ti3AlC2 film and n-Si show the expected rectification (diode) characteristics, in contrast to the ohmic contact behavior in the case of Ti3AlC2 on p-Si. A triboelectric-nanogenerator-based touch-sensing device, comprising of the Ti3AlC2 film, shows a very impressive peak-to-peak open-circuit output voltage of 80 V. These observations reveal that pulsed laser deposited Ti3AlC2 thin films have excellent potential for applications in multiple domains, such as bottom electrodes, resistors for high-precision measurements, Schottky diodes, ohmic contacts, fairly transparent ultrathin conductors, and next-generation biomechanical touch sensors for energy harvesting.",2007.04798v1 2022-01-19,Tearing instability and current-sheet disruption in the turbulent dynamo,"Turbulence in a conducting plasma can amplify seed magnetic fields in what is known as the turbulent, or small-scale, dynamo. The associated growth rate and emergent magnetic-field geometry depend sensitively on the material properties of the plasma, in particular on the Reynolds number ${\rm Re}$, the magnetic Reynolds number ${\rm Rm}$, and their ratio ${\rm Pm}\equiv{\rm Rm}/{\rm Re}$. For ${\rm Pm} > 1$, the amplified magnetic field is gradually arranged into a folded structure, with direction reversals at the resistive scale and field lines curved at the larger scale of the flow. As the mean magnetic energy grows to come into approximate equipartition with the fluid motions, this folded structure is thought to persist. Using analytical theory and high-resolution MHD simulations with the Athena++ code, we show that these magnetic folds become unstable to tearing during the nonlinear stage of the dynamo for ${\rm Rm}\gtrsim 10^4$ and ${\rm Re}\gtrsim 10^3$. An ${\rm Rm}$- and ${\rm Pm}$-dependent tearing scale, at and below which folds are disrupted, is predicted theoretically and found to match well the characteristic field-reversal scale measured in the simulations. The disruption of folds by tearing increases the ratio of viscous-to-resistive dissipation. In the saturated state, the magnetic-energy spectrum exhibits a sub-tearing-scale steepening to a slope consistent with that predicted for tearing-mediated Alfv\'enic turbulence. Its spectral peak appears to be independent of the resistive scale and comparable to the driving scale of the flow, while the magnetic energy resides in a broad range of scales extending down to the field-reversal scale set by tearing. Emergence of a degree of large-scale magnetic coherence in the saturated state of the turbulent dynamo may be consistent with observations of magnetic-field fluctuations in galaxy clusters and recent laboratory experiments.",2201.07757v2 2014-04-10,Metal-insulator transition upon heating and negative-differential-resistive-switching induced by self-heating in BaCo0.9Ni0.1S1.8,"The layered compound BaCo1-xNixS2-y (0.051.0T) and a relative high Curie temperature. This realization of robust QAH state in hard FMTIs is a major step towards dissipationless electronic applications without external fields.",1412.3758v2 2015-01-22,High spin polarization and large spin splitting in equiatomic quaternary CoFeCrAl Heusler alloy,"In this paper, we investigate CoFeCrAl alloy by means of various experimental techniques and ab-initio calculations to look for half-metallic nature. The alloy is found to exist in the cubic Heusler structure, with presence of B2 ordering. Saturation magnetization (MS) value of about 2 Bohr magneton/f.u. is observed at 8 K under ambient pressure, which is in good agreement with the Slater-Pauling rule. MS values are found to be independent of pressure, which is a prerequisite for half-metals. The ab-initio electronic structure calculations predict half-metallic nature for the alloy with a spin slitting energy of 0.31 eV. Importantly, this system shows a high current spin polarization value of 0.67 [with error of 0.02], as deduced from the point contact Andreev reflection (PCAR) measurements. Linear dependence of electrical resistivity with temperature indicates the possibility of reasonably high spin polarization at elevated temperatures (~150 K) as well. All these suggest that CoFeCrAl is a promising material for the spintronic devices.",1501.05599v1 2015-12-08,A Two-Temperature Model of Magnetized Protostellar Outflows,"We explore kinematics and morphologies of molecular outflows driven by young protostars using magnetohydrodynamic simulations in the context of the unified wind model of Shang et al. The model explains the observed high-velocity jet and low-velocity shell features. In this work we investigate how these characteristics are affected by the underlying temperature and magnetic field strength. We study the problem of a warm wind running into a cold ambient toroid by using a tracer field that keeps track of the wind material. While an isothermal equation of state is adopted, the effective temperature is determined locally based on the wind mass fraction. In the unified wind model, the density of the wind is cylindrically stratified and highly concentrated toward the outflow axis. Our simulations show that for a sufficiently magnetized wind, the jet identity can be well maintained even at high temperatures. However, for a high temperature wind with low magnetization, the thermal pressure of the wind gas can drive material away from the axis, making the jet less collimated as it propagates. We also study the role of the poloidal magnetic field of the toroid. It is shown that the wind-ambient interface becomes more resistant to corrugation when the poloidal field is present, and the poloidal field that bunches up within the toroid prevents the swept-up material from being compressed into a thin layer. This suggests that the ambient poloidal field may play a role in producing a smoother and thicker swept-up shell structure in the molecular outflow.",1512.02609v1 2017-10-25,Small-mass atomic defects enhance vibrational thermal transport at disordered interfaces with ultrahigh thermal boundary conductance,"The role of interfacial nonidealities and disorder on thermal transport across interfaces is traditionally assumed to add resistance to heat transfer, decreasing the thermal boundary conductance (TBC).$^1$ However, recent computational works have suggested that interfacial defects can enhance this thermal boundary conductance through emergence of unique vibrations that are intrinsic to the material interface and defect atoms,$^{2-6}$ a finding that contradicts traditional theory and conventional understanding. By manipulating the local heat flux of atomic vibrations that comprise these interfacial modes, in principle, the TBC can be increased. In this work, we provide evidence that interfacial defects can enhance the TBC across interfaces through the emergence of unique high frequency vibrational modes that arise from atomic mass defects at the interface with relatively small masses. We demonstrate ultrahigh TBC at amorphous SiOC:H/SiC:H interfaces, approaching 1 GW m$^{-2}$ K$^{-1}$, that is further increased through the introduction of nitrogen defects. The fact that disordered interfaces can exhibit such high conductances, which can be further increased with additional defects offers a unique direction in controlling interfacial thermal transport that becomes important in manipulating heat transfer across materials with high densities of interfaces.",1710.09440v1 2019-03-14,Nonsaturating large magnetoresistance in the high carrier density nonsymmorphic metal CrP,"The band structure of high carrier density metal CrP features an interesting crossing at the Y point of the Brillouin zone. The crossing, which is protected by the nonsymmorphic symmetry of the space group, results in a hybrid, semi-Dirac-like energy-momentum dispersion relation near Y. The linear energy-momentum dispersion relation along Y-$\Gamma$ is reminiscent of the observed band structure in several semimetallic extremely large magnetoresistance (XMR) materials. We have measured the transverse magnetoresistance of CrP up to 14 T at temperatures as low as $\sim$ 16 mK. Our data reveal a nonsaturating, quadratic magnetoresistance as well as the behaviour of the so-called `turn-on' temperature in the temperature dependence of resistivity. Despite the difference in the magnitude of the magnetoresistance and the fact that CrP is not a semimetal, these features are qualitatively similar to the observations reported for XMR materials. Thus, the high-field electrical transport studies of CrP offer the prospect of identifying the possible origin of the nonsaturating, quadratic magnetoresistance observed in a wide range of metals.",1903.05914v1 2018-07-03,An Inside Look at the Ti-MoS2 Contact in Ultra-thin Field Effect Transistor with Atomic Resolution,"Two-dimensional molybdenum disulfide (MoS2) is an excellent channel material for ultra-thin field effect transistors. However, high contact resistance across the metal-MoS2 interface continues to limit its widespread realization. Here, using atomic-resolution analytical scanning transmission electron microscopy (STEM) together with first principle calculations, we show that this contact problem is a fundamental limitation from the bonding and interactions at the metal-MoS2 interface that cannot be solved by improved deposition engineering. STEM analysis in conjunction with theory shows that when MoS2 is in contact with Ti, a metal with a high affinity to form strong bonds with sulfur, there is a release of S from Mo along with the formation of small Ti/TixSy clusters. A destruction of the MoS2 layers and penetration of metal can also be expected. The design of true high-mobility metal-MoS2 contacts will require the optimal selection of the metal or alloy based on their bonding interactions with the MoS2 surface. This can be advanced by evaluation of binding energies with increasing the number of atoms within metal clusters.",1807.01377v1 2021-02-03,Novel drying additives and their evaluation for self-flowing refractory castables,"The drying step of dense refractory castables containing hydraulic binders is a critical process, which usually requires using slow heating rates due to the high explosion trend of such materials during their first thermal treatment. Thus, this work investigated the performance of alternative additives to induce faster and safer drying of self-flowing high-alumina refractory castables bonded with calcium aluminate cement (CAC) or hydratable alumina (HA). The following materials were analyzed for this purpose: polymeric fibers, a permeability enhancing compound (RefPac MIPORE 20) and an organic additive (aluminum salt of 2-hydroxypropanoic acid). The drying behavior and explosion resistance of the cured samples were evaluated when subjecting the prepared castables to heating rates of 2, 5 or 20C/min and the obtained data were then correlated to the potential of the drying agents to improve the permeability and mechanical strength level of the refractories at different temperatures. The collected results attested that the selected additives were more efficient in optimizing the drying behavior of the CAC-bonded compositions, whereas the HA-containing castables performed better when the aluminum-based salt was blended with a small amount of CAC (0.5 wt.%), which changed the binders hydration reaction sequence and optimized the permeability level of the resulting microstructure. Consequently, some of the designed compositions evaluated in this work showed improved drying behavior and no explosion was observed even during the tests carried out under a high heating rate (20C/min).",2102.02008v1 2021-02-06,"Contact-Barrier Free, High Mobility, Dual-Gated Junctionless Transistor Using Tellurium Nanowire","Gate-all-around nanowire transistor, due to its extremely tight electrostatic control and vertical integration capability, is a highly promising candidate for sub-5 nm technology node. In particular, the junctionless nanowire transistors are highly scalable with reduced variability due to avoidance of steep source/drain junction formation by ion implantation. Here we demonstrate a dual-gated junctionless nanowire \emph{p}-type field effect transistor using tellurium nanowire as the channel. The dangling-bond-free surface due to the unique helical crystal structure of the nanowire, coupled with an integration of dangling-bond-free, high quality hBN gate dielectric, allows us to achieve a phonon-limited field effect hole mobility of $570\,\mathrm{cm^{2}/V\cdot s}$ at 270 K, which is well above state-of-the-art strained Si hole mobility. By lowering the temperature, the mobility increases to $1390\,\mathrm{cm^{2}/V\cdot s}$ and becomes primarily limited by Coulomb scattering. \txc{The combination of an electron affinity of $\sim$4 eV and a small bandgap of tellurium provides zero Schottky barrier height for hole injection at the metal-contact interface}, which is remarkable for reduction of contact resistance in a highly scaled transistor. Exploiting these properties, coupled with the dual-gated operation, we achieve a high drive current of $216\,\mathrm{\mu A/\mu m}$ while maintaining an on-off ratio in excess of $2\times10^4$. The findings have intriguing prospects for alternate channel material based next-generation electronics.",2102.03507v1 2021-05-27,Route to High-Performance Micro-solid Oxide Fuel Cells on Metallic Substrates,"Micro-solid oxide fuel cells based on thin films have strong potential for use in portable power devices. However, devices based on silicon substrates typically involve thin-film metallic electrodes which are unstable at high temperatures. Devices based on bulk metal substrates overcome these limitations, though performance is hindered by the challenge of growing state-of-the-art epitaxial materials on metals. Here, we demonstrate for the first time the growth of epitaxial cathode materials on metal substrates (stainless steel) commercially supplied with epitaxial electrolyte layers (1.5 {um (Y2O3)0.15(ZrO2)0.85 (YSZ) + 50 nm CeO2). We create epitaxial mesoporous cathodes of (La0.60Sr0.40)0.95Co0.20Fe0.80O3 (LSCF) on the substrate by growing LSCF/MgO vertically aligned nanocomposite films by pulsed laser deposition, followed by selectively etching out the MgO. To enable valid comparison with the literature, the cathodes are also grown on single-crystal substrates, confirming state-of-the-art performance with an area specific resistance of 100ohmegacm2 at 500dC and activation energy down to 0.97 eV. The work marks an important step toward the commercialization of high-performance micro-solid oxide fuel cells for portable power applications.",2105.13117v1 2023-03-15,Characterization of local deformation around hydrides in Zircaloy-4 using conventional and high angular resolution electron backscatter diffraction,"Zircaloy-4 is used as a fuel cladding material for water reactors, as it has good mechanical properties, corrosion resistance, and a low thermal neutron absorption cross section. However, the mechanical performance of Zircaloy-4 can be reduced during service due to hydrogen uptake and hydride formation. These hydrides are brittle, and often reduce the strength and toughness of materials as well as increase susceptibility to delayed hydride cracking (DHC). In this work, large grain Zircaloy-4 with hydrides was prepared and then cross sectioned using cryo-ion beam polishing, using plasma focused ion beam (pFIB) and broad ion beam (BIB) approaches to enable the preparation of a very high quality flat surface with no preferential etching of either the hydride or zirconium metal (typically metallographic polishing preferentially removes hydrides). Conventional and high angular resolution electron backscatter diffraction (EBSD) analysis were then used to explore morphology, deformation fields, and orientation relationships between the zirconium matrix and hydrides. Four maps were collected for analysis which included hydrides near grain boundaries: (a) where the hydride smoothly decorates across two of the connecting boundaries near a triple junction; (b) where the hydride smoothly decorates the boundary; (c) a mixture of smooth decoration of the interface and protrusion into the grains; (d) fine scale hydride that protrudes into one grain. This work highlights that incompatibility of the hydride within the zirconium matrix is strongly linked to the orientation relationship of the hydride and matrix, and the grain boundary character. These results may enable enhanced understanding of the role of hydrides in fracture as well as stress-induced hydride reorientation and DHC susceptibility.",2303.08311v1 2014-10-15,Cyclic Strength and Nonlinear Material Fracture Mechanics (by the example of steels),"It was shown that a material fatigue fracture diagram can be viewed as a locus of points with $\sigma $ and $\sqrt l$ coordinates' product equal to $K_{1c}/2$, and $\sigma $ and $l$ product -- to $G_{1c}/2$, where $K_{1c}$ and $G_{1c}$ are non-linear fracture mechanics force and energy criteria. It was established that the average number of interatomic bonds destroyed within one alternate stress $\nabla_{1cs}$ cycle is directly proportional to $\sigma $ that is twice as large as a peak value of $\sigma^a$. It was found that low-cycle fatigue is characterized by $\sigma >\sigma_{0.2}$ and $\sigma_{1cs}> 1$, high-cycle fatigue -- by $\sigma = \sigma_{0.2}$ and $\nabla_{1cs} = 1$, and giga-cycle fatigue -- by $\sigma < \sigma_{0.2}$ and $\nabla_{1cs} < 1$. An individual interatomic bond cannot be destroyed part by part but as a single unit. The latter means that in giga-cycle fatigue a single interatomic bond is destroyed within several cycles rather than within a single cycle. The factors $F$ (collapsibility) and $R$ (resistibility) were proposed and mentioned as essential material physical constants. The introduced notion $\nabla_{1cs}$ and the established linear nature of $\nabla_{1cs}$ relationship allow to: a) clarify the fatigue crack growth physical nature in low-, high- and giga-cycle fracture zones; b) determine the nature of a fatigue fracture diagram disruption; c) plot the fatigue fracture diagram using the results obtained in a single specimen cyclic strength test with a selected value of $\sigma \ge \sigma_{0.2}$. For giga-cycle fatigue it is important (with similar purpose in mind) to determine this dependence for $\sigma < \sigma_{0.2}$. It is recommended to use $G_{1c}$ criterion to find the $l_{cr}$ length value which in contrast to $K_{1c}$ has a clear physical nature.",1410.4177v2 2014-12-14,Gate-tunable quantum oscillations in ambipolar Cd3As2 thin films,"Electrostatic doping in materials can lead to various exciting electronic properties, such as metal-insulator transition and superconductivity, by altering the Fermi level position or introducing exotic phases. Cd3As2, a three-dimensional (3D) analog of graphene with extraordinary carrier mobility, was predicted to be a 3D Dirac semimetal, a feature confirmed by recent experiments. However, most research so far has been focused on metallic bulk materials that are known to possess ultra-high mobility and giant magnetoresistance but limited carrier transport tunability. Here, we report on the first observation of a gate-induced transition from band conduction to hopping conduction in single-crystalline Cd3As2 thin films via electrostatic doping by solid electrolyte gating. The extreme charge doping enables the unexpected observation of p-type conductivity in a 50 nm-thick Cd3As2 thin film grown by molecular beam epitaxy. More importantly, the gate-tunable Shubnikov-de Haas (SdH) oscillations and the temperature-dependent resistance reveal a unique band structure and bandgap opening when the dimensionality of Cd3As2 is reduced. This is also confirmed by our first-principles calculations. The present results offer new insights towards nanoelectronic and optoelectronic applications of Dirac semimetals in general, and provide new routes in the search for the intriguing quantum spin Hall effect in low-dimension Dirac semimetals, an effect that is theoretically predicted but not yet experimentally realized.",1412.4380v2 2016-05-15,Nearly massless Dirac fermions hosted by Sb square net in BaMnSb2,"Layered compounds AMnBi2 (A=Ca, Sr, Ba, or rare earth element) have been established as Dirac materials. Dirac electrons generated by the two-dimensional (2D) Bi square net in these materials are normally massive due to the presence of a spin-orbital coupling (SOC) induced gap at Dirac nodes. Here we report that the Sb square net in an isostructural compound BaMnSb2 can host nearly massless Dirac fermions. We observed strong Shubnikov-de Haas (SdH) oscillations in this material. From the analyses of the SdH oscillations, we find key signatures of Dirac fermions, including light effective mass (~0.052m0; m0, mass of free electron), high quantum mobility (1280 cm2V-1S-1) and a Pi Berry phase accumulated along cyclotron orbit. Compared with AMnBi2, BaMnSb2 also exhibits much more significant quasi two-dimensional (2D) electronic structure, with the out-of-plane transport showing nonmetallic conduction below 120K and the ratio of the out-of-plane and in-plane resistivity reaching ~670. Additionally, BaMnSb2 also exhibits an antiferromagnetic order with a weak ferromagnetic component. The combination of nearly massless Dirac fermions on quasi-2D planes with a magnetic order makes BaMnSb2 an intriguing platform for seeking novel exotic phenomena of massless Dirac electrons.",1605.04613v2 2017-10-09,Huge magnetoresistance and ultra-sharp metamagnetic transition in polycrystalline ${Sm_{0.5}Ca_{0.25}Sr_{0.25}MnO_3}$,"Large magnetoresistive materials are of immense interest for a number of spintronic applications by developing high density magnetic memory devices, magnetic sensors and magnetic switches. Colossal magnetoresistance, for which resistivity changes several order of magnitude (${\sim10^4 \%}$) in an external magnetic field, occurs mainly in phase separated oxide materials, namely manganites, due to the phase competition between the ferromagnetic metallic and the antiferromagnetic insulating regions. Can one further enhance the magnetoresistance by tuning the volume fraction of the two phases? In this work, we report a huge colossal magnetoresistance along with the ultra-sharp metamagnetic transition in half doped ${Sm_{0.5}Ca_{0.25}Sr_{0.25}MnO_3}$ manganite compound by suitably tuning the volume fraction of the competing phases. The obtained magnetoresistance value at 10 K is as large as $\sim10^{13}\%$ in a 30 kOe external magnetic field and $\sim10^{15}\%$ in 90 kOe external magnetic field and is several orders of magnitude higher than any other observed magnetoresistance value reported so far. Using model Hamiltonian calculations we have shown that the inhomogeneous disorder, deduced from tunneling electron microscopy, suppresses the CE-type phase and seeds the ferromagnetic metal in an external magnetic field.",1710.03007v2 2018-09-12,V$_5$S$_8$: a Kondo lattice based on intercalation of van der Waals layered transition metal dichalcogenide,"Since the discovery of graphene, a tremendous amount of two dimensional (2D) materials have surfaced. Their electronic properties can usually be well understood without considering correlations between electrons. On the other hand, strong electronic correlations are known to give rise to a variety of exotic properties and new quantum phases, for instance, high temperature superconductivity, heavy fermions and quantum spin liquids. The study of these phenomena has been one of the main focuses of condensed matter physics. There is a strong incentive to introduce electronic correlations into 2D materials. Via intercalating a van der Waals layered compound VS$_2$, we show an emergence of a Kondo lattice, an extensively studied strongly correlated system, by magnetic, specific heat, electrical and thermoelectric transport studies. In particular, an exceptionally large Sommerfeld coefficient, 440 mJ$\cdot$K$^{-2}\cdot$mol$^{-1}$, indicates a strong electron correlation. The obtained Kadowaki-Woods ratio, $2.7\times 10^{-6}$ $\mu\Omega\cdot$cm$\cdot$mol$^2\cdot$K$^2\cdot$mJ$^{-2}$, also supports the strong electron-electron interaction. The temperature dependence of the resistivity and thermopower corroborate the Kondo lattice picture. The intercalated compound is one of a few rare examples of $d$-electron Kondo lattices. We further show that the Kondo physics persists in ultra-thin films. This work thus demonstrates a route to generate strong correlations in 2D materials.",1809.04213v1 2014-08-03,"Carrier screening, transport, and relaxation in 3D Dirac semimetals","A theory is developed for the density and temperature dependent carrier conductivity in doped three-dimensional (3D) Dirac materials focusing on resistive scattering from screened Coulomb disorder due to random charged impurities (e.g., dopant ions and unintentional background impurities). The theory applies both in the undoped intrinsic (""high-temperature"", $T \gg T_F$) and the doped extrinsic (""low-temperature"", $T \ll T_F$) limit with analytical scaling properties for the carrier conductivity obtained in both regimes, where $T_F$ is the Fermi temperature corresponding to the doped free carrier density (electrons or holes). The scaling properties describing how the conductivity depends on the density and temperature can be used to establish the Dirac nature of 3D systems through transport measurements. We also consider the temperature dependent conductivity limited by the acoustic phonon scattering in 3D Dirac materials. In addition, we theoretically calculate and compare the single particle relaxation time $\tas$, defining the quantum level broadening, and the transport scattering time $\tat$, defining the conductivity, in the presence of screened charged impurity scattering. A critical quantitative analysis of the $\tat/\tas$ results for 3D Dirac materials in the presence of long-range screened Coulomb disorder is provided.",1408.0518v2 2017-03-28,Metallic vanadium disulfide nanosheets as a platform material for multifunctional electrode applications,"Nano-thick metallic transition metal dichalcogenides such as VS$_{2}$ are essential building blocks for constructing next-generation electronic and energy-storage applications, as well as for exploring unique physical issues associated with the dimensionality effect. However, such 2D layered materials have yet to be achieved through either mechanical exfoliation or bottom-up synthesis. Herein, we report a facile chemical vapor deposition route for direct production of crystalline VS$_{2}$ nanosheets with sub-10 nm thicknesses and domain sizes of tens of micrometers. The obtained nanosheets feature spontaneous superlattice periodicities and excellent electrical conductivities (~3$\times$10$^{3}$ S cm$^{-1}$), which has enabled a variety of applications such as contact electrodes for monolayer MoS$_{2}$ with contact resistances of ~1/4 to that of Ni/Au metals, and as supercapacitor electrodes in aqueous electrolytes showing specific capacitances as high as 8.6$\times$10$^{2}$ F g$^{-1}$. This work provides fresh insights into the delicate structure-property relationship and the broad application prospects of such metallic 2D materials.",1703.09582v1 2019-02-26,Superconductivity at 161 K in Thorium Hydride $ThH_{10}$: Synthesis and Properties,"Here we report targeted high-pressure synthesis of two novel high-$T_C$ hydride superconductors, $P6_3/mmc$-$ThH_9$ and $Fm\bar{3}m$-$ThH_{10}$, with the experimental critical temperatures ($T_C$) of 146 K and 159-161 K and upper critical magnetic fields ($\mu$$H_C$) 38 and 45 Tesla at pressures 170-175 Gigapascals, respectively. Superconductivity was evidenced by the observation of zero resistance and a decrease of $T_C$ under external magnetic field up to 16 Tesla. This is one of the highest critical temperatures that has been achieved experimentally in any compounds, along with such materials as $LaH_{10}$, $H_3S$ and $HgBa_2Ca_xCu_2O_{6+z}$. Our experiments show that $fcc$-$ThH_{10}$ has stabilization pressure of 85 GPa, making this material unique among all known high-$T_C$ metal polyhydrides. Two recently predicted Th-H compounds, $I4/mmm$-$ThH_4$ (> 86 GPa) and $Cmc2_1$-$ThH_6$ (86-104 GPa), were also synthesized. Equations of state of obtained thorium polyhydrides were measured and found to perfectly agree with the theoretical calculations. New phases were examined theoretically and their electronic, phonon, and superconducting properties were calculated.",1902.10206v4 2022-02-10,"Giant magnetoresistance, Fermi surface topology, Shoenberg effect and vanishing quantum oscillations in type-II Dirac semimetal candidates MoSi$_2$ and WSi$_2$","We performed comprehensive theoretical and experimental studies of the electronic structure and the Fermi surface topology of two novel quantum materials, MoSi$_2$ and WSi$_2$. The theoretical predictions of the electronic structure in the vicinity of the Fermi level was verified experimentally by thorough analysis of the observed quantum oscillations in both electrical resistivity and magnetostriction. We established that the Fermi surface sheets in MoSi$_2$ and WSi$_2$ consist of 3D dumbbell-shaped hole-like pockets and rosette-shaped electron-like pockets, with nearly equal volumes. Based on this finding, both materials were characterized as almost perfectly compensated semimetals. In conjunction, the magnetoresistance attains giant values of $10^4$ and $10^5\,\%$ for WSi$_2$ and MoSi$_2$, respectively. In turn, the anisotropic magnetoresistance achieves $-95$ and $-98\,\%$ at $T=2\,$K and in $B=14\,$T for WSi$_2$ and MoSi$_2$, respectively. Furthermore, for both compounds we observed the Shoenberg effect in their Shubnikov-de Haas oscillations that persisted at as high temperature as $T=25\,$K in MoSi$_2$ and $T=12\,$K in WSi$_2$. In addition, we found for MoSi$_2$ a rarely observed spin-zero phenomenon. Remarkably, the electronic structure calculations revealed type-II Dirac cones located near 480 meV and 710 meV above the Fermi level in MoSi$_2$ and WSi$_2$, respectively.",2202.05362v1 2017-04-24,1D van der Waals Material Tellurium: Raman Spectroscopy under Strain and Magneto-transport,"Experimental demonstrations of 1D van der Waals material tellurium have been presented by Raman spectroscopy under strain and magneto-transport. Raman spectroscopy measurements have been performed under strains along different principle axes. Pronounced strain response along c-axis is observed due to the strong intra-chain covalent bonds, while no strain response is obtained along a-axis due to the weak inter-chain van der Waals interaction. Magneto-transport results further verify its anisotropic property, resulting in dramatically distinct magneto-resistance behaviors in terms of three different magnetic field directions. Specifically, phase coherence length extracted from weak antilocalization effect, L$_{\Phi}$ ~ T$^{-0.5}$, claims its 2D transport characteristics when an applied magnetic field is perpendicular to the thin film. In contrast, L$_{\Phi}$ ~ T$^{-0.33}$ is obtained from universal conductance fluctuations once the magnetic field is along c-axis of Te, indicating its nature of 1D transport along the helical atomic chains. Our studies, which are obtained on high quality single crystal tellurium thin film, appear to serve as strong evidences of its 1D van der Waals structure from experimental perspectives. It is the aim of this paper to address this special concept that differs from the previous well-studied 1D nanowires or 2D van der Waals materials.",1704.07020v1 2019-03-09,A New Magnetic Topological Quantum Material Candidate by Design,"Magnetism, when combined with an unconventional electronic band structure, can give rise to forefront electronic properties such as the quantum anomalous Hall effect, axion electrodynamics, and Majorana fermions. Here we report the characterization of high-quality crystals of EuSn$_2$P$_2$, a new quantum material specifically designed to engender unconventional electronic states plus magnetism. EuSn$_2$P$_2$ has a layered, Bi$_2$Te$_3$-type structure. Ferromagnetic interactions dominate the Curie-Weiss susceptibility, but a transition to antiferromagnetic ordering occurs near 30 K. Neutron diffraction reveals that this is due to two-dimensional ferromagnetic spin alignment within individual Eu layers and antiferromagnetic alignment between layers - this magnetic state surrounds the Sn-P layers at low temperatures. The bulk electrical resistivity is sensitive to the magnetism. Electronic structure calculations reveal that EuSn$_2$P$_2$ might be a strong topological insulator, which can be a new magnetic topological quantum material (MTQM) candidate. The calculations show that surface states should be present, and they are indeed observed by ARPES measurements.",1903.03888v1 2019-01-23,Enhancing Interconnect Reliability and Performance by Converting Tantalum to 2D Layered Tantalum Sulfide at Low Temperature,"The interconnect half-pitch size will reach ~20 nm in the coming sub-5 nm technology node. Meanwhile, the TaN/Ta (barrier/liner) bilayer stack has to be > 4 nm to ensure acceptable liner and diffusion barrier properties. Since TaN/Ta occupy a significant portion of the interconnect cross-section and they are much more resistive than Cu, the effective conductance of an ultra-scaled interconnect will be compromised by the thick bilayer. Therefore, two dimensional (2D) layered materials have been explored as diffusion barrier alternatives. However, many of the proposed 2D barriers are prepared at too high temperatures to be compatible with the back-end-of-line (BEOL) technology. In addition, as important as the diffusion barrier properties, the liner properties of 2D materials must be evaluated, which has not yet been pursued. Here, a 2D layered tantalum sulfide (TaSx) with ~1.5 nm thickness is developed to replace the conventional TaN/Ta bilayer. The TaSx ultra-thin film is industry-friendly, BEOL-compatible, and can be directly prepared on dielectrics. Our results show superior barrier/liner properties of TaSx compared to the TaN/Ta bilayer. This single-stack material, serving as both a liner and a barrier, will enable continued scaling of interconnects beyond 5 nm node.",1901.08143v1 2020-08-31,Enhanced fracture toughness in ceramic superlattice thin films: on the role of coherency stresses and misfit dislocations,"Superlattice (SL) thin films composed of refractory ceramics unite extremely high hardness and enhanced fracture toughness; a material combination often being mutually exclusive. While the hardness enhancement obtained whentwo materials form a superlattice is well described by existing models based on dislocation mobility, the underlying mechanisms behind the increase in fracture toughness are yet to be unraveled. Here we provide a model based on linear elasticity theory to predict the fracture toughness enhancement in (semi-)epitaxial nanolayers due to coherency stresses and formation of misfit dislocations. We exemplarily study a superlattice structure composed of two cubic transition metal nitrides (TiN, CrN) on a MgO (100) single-crystal substrate. Minimization of the overall strain energy, each time a new layer is added on the nanolayered stack, allows estimating the density of misfit dislocations formed at the interfaces. The evolving coherency stresses, which are partly relaxed by the misfit dislocations, are then used to calculate the apparent fracture toughness of respective SL architectures by applying the weight function method. The results show that the critical stress intensity increases steeply with increasing bilayer period for very thin (essentially dislocation-free) SLs, before the K_IC values decline more gently along with the formation of misfit dislocations. The characteristic K_IC vs. bilayer-period-dependence nicely matches experimental trends. Importantly, all critical stress intensity values of the superlattice films clearly exceed the intrinsic fracture toughness of the constituting layer materials, evincing the importance of coherency stresses for increasing the crack growth resistance.",2008.13652v1 2020-12-10,Evidence of non-trivial Berry phase and Kondo physics in SmBi,"Realization of semimetals with non-trivial topologies such as Dirac and Weyl semimetals, have provided a boost in the study of these quantum materials. Presence of electron correlation makes the system even more exotic due to enhanced scattering of charge carriers, Kondo screening etc. Here, we studied the electronic properties of single crystalline, SmBi employing varied state of the art bulk measurements. Magnetization data reveals two magnetic transitions; an antiferromagnetic order with a Neel temperature of ~ 9 K and a second magnetic transition at a lower temperature (= 7 K). The electrical resistivity data shows an upturn typical of a Kondo system and the estimated Kondo temperature is found to be close to the Neel temperature. High quality of the crystal enabled us to discover signature of quantum oscillation in the magnetization data even at low magnetic field. Using a Landau level fan diagram analysis, a non-trivial Berry phase is identified for a Fermi pocket revealing the topological character in this material. These results demonstrate an unique example of the Fermiology in the antiferromagnetic state and opens up a new paradigm to explore the Dirac fermion physics in correlated topological metal via interplay of Kondo interaction, topological order and magnetism.",2012.05459v1 2021-03-25,Bonding nature and optical contrast of $TiTe_2$/$Sb_2Te_3$ phase-change heterostructure,"Chalcogenide phase-change materials (PCMs) are regarded as the leading candidate for storage-class non-volatile memory and neuro-inspired computing. Recently, using the $TiTe_2$/$Sb_2Te_3$ material combination, a new framework - phase-change heterostructure (PCH), has been developed and proved to effectively suppress the noise and drift in electrical resistance upon memory programming, largely reducing the inter-device variability. However, the atomic-scale structural and chemical nature of PCH remains to be fully understood. In this work, we carry out thorough ab initio simulations to assess the bonding characteristics of the PCH. We show that the $TiTe_2$ crystalline nanolayers do not chemically interact with the surrounding $Sb_2Te_3$, and are stabilized by strong covalent and electrostatic Ti-Te interactions, which create a prohibitively high barrier for atomic migrations along the pulsing direction. We also find significant contrast in computed dielectric functions in the PCH, suggesting possible optical applications of this class of devices. With the more confined space and therefore constrained phase transition compared to traditional PCM devices, the recently introduced class of PCH-based devices may lead to improvements in phase-change photonic and optoelectronic applications with much lower stochasticity during programming.",2103.13583v2 2021-06-30,Classifying charge carrier interaction in highly-compressed elements and silane,"Since pivotal experimental discovery of the near-room-temperature superconductivity (NRTS) in highly-compressed sulphur hydride by Drozdov et al (2015 Nature 525 73-76), more than a dozen of binary and of ternary hydrogen-rich phases exhibited superconducting transition above 100 K have been discovered to date. There is a widely accepted theoretical point of view that primary mechanism governing the emergence of superconductivity in hydrogen-rich phases is the electron-phonon pairing. However, our recent analysis of experimental temperature dependent resistance in $H_{3}S$, $LaH_{x}$, $PrH_{9}$ and $BaH_{12}$ (arXiv: 2104.14145) showed that these compounds exhibit the dominance of non-electron-phonon charge carrier interaction and, thus, it is unlikely that the electron-phonon pairing is the primary mechanism for the emergence of superconductivity in these materials. Here we use the same approach to reveal charge carrier interaction in highly-compressed lithium, black phosphorous, sulfur, and silane. We found that all these superconductors exhibit the dominance of non-electron-phonon charge carrier interaction. This explains the failure of high-Tc values predicted for these materials by the first-principles calculations which utilized the electron-phonon pairing as the mechanism for the emergence of superconductivity in these materials. Our result implies that alternative pairing mechanisms (i.e., electron-magnon, electron-polaron, electron-electron, etc.) should be tested within first-principles calculations approach as possible mechanisms for the emergence of superconductivity in highly-compressed superconductors.",2106.15873v1 2021-09-08,Coherent spin rotation-induced zero thermal expansion in MnCoSi-based spiral magnets,"Materials exhibiting zero thermal expansion (ZTE), namely, volume invariance during temperature change, can resist thermal shock and are highly desired in modern industries as high-precision components. However, pure ZTE materials are rare, especially those that are metallic. Here, we report the discovery of a pure metallic ZTE material: an orthorhombic Mn1-xNixCoSi spiral magnet. The introduction of Ni can efficiently enhance the ferromagnetic exchange interaction and construct the transition from a spiral magnetic state to a ferromagnetic-like state in MnCoSi-based alloys. Systematic in situ neutron powder diffraction revealed a new cycloidal spiral magnetic structure in bc plane at ground state which would transform to the helical spiral in the ab plane with increasing temperature. Combined with Lorentz transmission electron microscopy techniques, the cycloidal and helical spin order coherently rotated at varying periods along the c axis during the magnetic transition. This spin rotation drove the continuous movement of the coupled crystalline lattice and induced a large negative thermal expansion along the a axis, eventually leading to a wide-temperature ZTE effect. Our work not only introduces a new ZTE alloy but also presents a new mechanism by which to discover or design ZTE magnets.",2109.03557v1 2022-04-09,Role of substrate surface morphology on the performance of graphene inks for flexible electronics,"Two-dimensional (2D) materials, such as graphene, are seen as potential candidates for fabricating electronic devices and circuits on flexible substrates. Inks or dispersions of 2D materials can be deposited on flexible substrates by large-scale coating techniques, such as inkjet printing and spray coating. One of the main issues in coating processes is nonuniform deposition of inks, which may lead to large variations of properties across the substrates. Here, we investigate the role of surface morphology on the performance of graphene ink deposited on different paper substrates with specific top coatings. Substrates with good wetting properties result in reproducible thin films and electrical properties with low sheet resistance. The correct choice of surface morphology enables high-performance films without postdeposition annealing or treatment. Scanning terahertz time-domain spectroscopy (THz-TDS) is introduced to evaluate both the uniformity and the local conductivity of graphene inks on paper. A paper-based strain gauge is demonstrated and a variable resistor acts as an on-off switch for operating an LED. Customized surfaces can thus help in unleashing the full potential of ink-based 2D materials.",2204.04503v1 2023-04-28,"First-principles Prediction of Potential Candidate Materials MCu$_3$X$_4$ (M = V, Nb, Ta; X = S, Se, Te) for Neuromorphic Computing","Inspired by the neuro-synaptic frameworks in the human brain, neuromorphic computing is expected to overcome the bottleneck of traditional von-Neumann architecture and be used in artificial intelligence. Here, we predict a class of potential candidate materials, MCu$_3$X$_4$ (M = V, Nb, Ta; X = S, Se, Te), for neuromorphic computing applications through first-principles calculations based on density functional theory. We find that when MCu$_3$X$_4$ are inserted with Li atom, the systems would transform from semiconductors to metals due to the considerable electron filling [~0.8 electrons per formula unit (f.u.)] and still maintain well structural stability. Meanwhile, the inserted Li atom also has a low diffusion barrier (~0.6 eV/f.u.), which ensures the feasibility to control the insertion/extraction of Li by gate voltage. These results establish that the system can achieve the reversible switching between two stable memory states, i.e., high/low resistance state, indicating that it could potentially be used to design synaptic transistor to enable neuromorphic computing. Our work provides inspiration for advancing the search of candidate materials related to neuromorphic computing from the perspective of theoretical calculations.",2304.14897v1 2023-06-26,Microscopic conductivity of passive films on ferritic stainless steel for hydrogen fuel cells,"Hydrogen fuel cells offer a clean and sustainable energy conversion solution. The bipolar separator plate, a critical component in fuel cells, plays a vital role in preventing reactant gas cross-contamination and facilitating efficient ion transport in a fuel cell. High chromium ferritic stainless steel with an artificially formed thin chromium oxide passive film has recently gained attention due to its superior electrical conductivity and corrosion resistance, making it a suitable material for separators. In this study, we investigate the microscopic electrical conductivity of the intrinsic passive oxide film on such ferritic stainless steel. Through advanced surface characterization techniques such as current sensing atomic force microscopy and scanning tunneling microscopy/spectroscopy, we discover highly conductive regions within the film that vary depending on location. These findings provide valuable insights into the behavior of the passive oxide film in fuel cells. By understanding the microscopic electrical properties, we can enhance the design and performance of separator materials in hydrogen fuel cells. Ultimately, this research contributes to a broader understanding of separator materials and supports the wider application of hydrogen fuel cells.",2306.14513v1 2003-10-20,Radiation induced oscillatory Hall effect in high mobility GaAs/AlGaAs devices,"We examine the radiation induced modification of the Hall effect in high mobility GaAs/AlGaAs devices that exhibit vanishing resistance under microwave excitation. The modification in the Hall effect upon irradiation is characterized by (a) a small reduction in the slope of the Hall resistance curve with respect to the dark value, (b) a periodic reduction in the magnitude of the Hall resistance, $R_{xy}$, that correlates with an increase in the diagonal resistance, $R_{xx}$, and (c) a Hall resistance correction that disappears as the diagonal resistance vanishes.",0310474v2 2015-09-03,A simple model for in- and out-of-plane resistivities of hole doped cuprates,"The highly anisotropic and qualitatively different nature of in- and out-of-plane charge dynamics in high-Tc cuprates cannot be accommodated within the conventional Boltzmann transport theory. The variation of in- and out-of-plane resistivities with temperature and hole content are also anomalous and cannot be explained by Fermi-liquid theory. In this study we have proposed a simple phenomenological model for the dc resistivity of cuprates by incorporating two firmly established generic features of all hole doped cuprate superconductors- (1) the pseudogap in the quasiparticle energy spectrum and (2) the T-linear resistivity at high temperatures. This T-linear behavior over an extended temperature range can be attributed to a quantum criticality, affecting the electronic phase diagram of cuprates. Experimental in-plane and out-of-plane resistivities of double layer Y(Ca)123 have been analyzed using the proposed model. This phenomenological model describes the temperature and hole content dependent resistivity over a wide range of temperature and hole content.",1509.01107v2 2015-10-12,The Mott-Ioffe-Regel limit and resistivity crossover in a tractable electron-phonon model,"Many metals display resistivity saturation - a substantial decrease in the slope of the resistivity as a function of temperature, that occurs when the electron scattering rate $\tau^{-1}$ becomes comparable to the Fermi energy $E_F/\hbar$ (the Mott-Ioffe-Regel limit). At such temperatures, the usual description of a metal in terms of ballistically propagating quasiparticles is no longer valid. We present a tractable model of a large $N$ number of electronic bands coupled to $N^2$ optical phonon modes, which displays a crossover behavior in the resistivity at temperatures where $\tau^{-1}\sim E_F/\hbar$. At low temperatures, the resistivity obeys the familiar linear form, while at high temperatures, the resistivity still increases linearly, but with a modified slope (that can be either lower or higher than the low-temperature slope, depending on the band structure). The high temperature non-Boltzmann regime is interpreted by considering the diffusion constant and the compressibility, both of which scale as the inverse square root of the temperature.",1512.00041v2 2022-02-13,Information Density in Multi-Layer Resistive Memories,"Resistive memories store information in a crossbar arrangement of two-terminal devices that can be programmed to patterns of high or low resistance. While extremely compact, this technology suffers from the ""sneak-path"" problem: certain information patterns cannot be recovered, as multiple low resistances in parallel make a high resistance indistinguishable from a low resistance. In this paper, a multi-layer device is considered, and the number of bits it can store is derived exactly and asymptotic bounds are developed. The information density of a series of isolated arrays with extreme aspect ratios is derived in the single- and multi-layer cases with and without peripheral selection circuitry. This density is shown to be non-zero in the limit, unlike that of the arrays with moderate aspect ratios previously considered. A simple encoding scheme that achieves capacity asymptotically is presented.",2202.06367v1 2023-09-27,Fractal-like star-mesh transformations using graphene quantum Hall arrays,"A mathematical approach is adopted for optimizing the number of total device elements required for obtaining high effective quantized resistances in graphene-based quantum Hall array devices. This work explores an analytical extension to the use of star-mesh transformations such that fractal-like, or recursive, device designs can yield high enough resistances (like 1 E{\Omega}, arguably the highest resistance with meaningful applicability) while still being feasible to build with modern fabrication techniques. Epitaxial graphene elements are tested, whose quantized Hall resistance at the nu=2 plateau (R_H = 12906.4 {\Omega}) becomes the building block for larger effective, quantized resistances. It is demonstrated that, mathematically, one would not need more than 200 elements to achieve the highest pertinent resistances",2309.15813v1 1999-01-25,Charge Transport in Synthetic Metals,"The phenomenology of charge transport in synthetic metals is reviewed. It is argued that the conventional quasiparticle picture and Boltzmann transport theory do not apply to these materials. The central ideas of Fermi liquid theory are reviewed, and the significant corrections produced by quasiparticle scattering from ferromagnetic spin fluctuations in liquid $^3$He are described. It is shown that Sr$_2$RuO$_4$ does not display the symptoms of a nearly-ferromagnetic Fermi liquid, so the source of its odd angular momentum pairing remains to be understood. The solution of an assisted-tunneling model of charge transport in quasi-one dimensional materials is described. This model has a quantum critical point and gives a resistivity that is linear in temperature or frequency, whichever is greater.",9901270v1 2000-01-11,Interpretation of a microwave induced current step in a single intrinsic Josephson junction on a Bi-2223 thin film,"Thin stacks consisting of a single intrinsic Josephson junction on (Bi,Pb)-Sr-Ca-Cu-O thin films are investigated under the influence of external microwave fields. The $I$-$V$-characteristic shows a single resistive branch, a clear superconducting gap edge structure and a pronounced current step in external microwave fields. With increasing irradiation power it shifts to higher voltages, while the height of the step remains practically unchanged. In a numerical simulation including an ac-magnetic field parallel to the superconducting layers the experimental features of the structure can be explained by a collective motion of Josephson fluxons.",0001152v2 2000-12-07,Superconductivity on the threshold of magnetism in CePd2Si2 and CeIn3,"The magnetic ordering temperature of some rare earth based heavy fermion compounds is strongly pressure-dependent and can be completely suppressed at a critical pressure, p$_c$, making way for novel correlated electron states close to this quantum critical point. We have studied the clean heavy fermion antiferromagnets CePd$_2$Si$_2$ and CeIn$_3$ in a series of resistivity measurements at high pressures up to 3.2 GPa and down to temperatures in the mK region. In both materials, superconductivity appears in a small window of a few tenths of a GPa on either side of p$_c$. We present detailed measurements of the superconducting and magnetic temperature-pressure phase diagram, which indicate that superconductivity in these materials is enhanced, rather than suppressed, by the closeness to magnetic order.",0012118v1 2002-02-03,Giant change in IR light transmission in La_{0.67}Ca_{0.33}MnO_{3} film near the Curie temperature: promising application in optical devices,"Transport, magnetic, magneto-optical (Kerr effect) and optical (light absorption) properties have been studied in an oriented polycrystalline La_{0.67}Ca_{0.33}MnO_{3} film which shows colossal magneto-resistance. The correlations between these properties are presented. A giant change in IR light transmission (more than a 1000-fold decrease) is observed on crossing the Curie temperature (about 270 K) from high to low temperature. Large changes in transmittance in a magnetic field were observed as well. The giant changes in transmittance and the large magneto-transmittance can be used for development of IR optoelectronic devices controlled by thermal and magnetic fields. Required material characteristics of doped manganites for these devices are discussed.",0202041v1 2002-07-10,Crystal growth and characterization of MgB2: Relation between structure and superconducting properties,"We discuss the important aspects of synthesis and crystal growth of MgB2 under high pressure (P) and temperature (T) in Mg-B-N system, including the optimisation of P-T conditions for reproducible crystal growth, the role of liquid phases in this process, the temperature dependence of crystal size and the effect of growing instabilities on single crystals morphology. Extensive experiments have been carried out on single crystals with slightly different lattice constants and defects concentration, which revealed and possible effects of Mg-deficiency and lattice strain on the superconducting properties of MgB2 (Tc, Jc, residual resistivity ratio, anisotropy etc.).",0207247v1 2002-07-10,Synthesis effects on the magnetic and superconducting properties of RuSr2GdCu2O8,"A systematic study on the synthesis of the Ru-1212 compound by preparing a series of samples that were annealed at increasing temperatures and then quenched has been performed. It results that the optimal temperature for the annealing lies around 1060-1065 C; a further temperature increase worsens the phase formation. Structural order is very important and the subsequent grinding and annealing improves it. Even if from the structural point of view the samples appear substantially similar, the physical characterization highlight great differences both in the electrical and magnetic properties related to intrinsic properties of the phase as well as to the connection between the grains as inferred from the resistive and the Curie Weiss behaviour at high temperature as well as in the visibility of ZFC anf FC magnetic signals.",0207265v1 2002-08-02,Transport spin polarisation in SrRuO3 measured through Point Contact Andreev reflection,"We report a study in which Andreev reflection using a Nb point contact is used to measure the transport spin polarisation of the 4d itinerant ferromagnet SrRuO3. By performing the study in high quality thin films with residual resistivities less than 7micro-ohm-cm, we ensure that the study is done in the ballistic limit, a regime which is difficult to reach in oxide ferromagnets. The degree of transport spin polarisation that we find is comparable to that of the hole doped rare-earth manganites. We conclude that the large transport spin polarisation results mainly from a difference in the Fermi velocities between the majority and minority spin channels in this material.",0208044v3 2002-08-23,Superconductivity in molecular solids with Jahn-Teller phonons,"We analyze fulleride superconductivity at experimental doping levels, treating the electron-electron and electron-phonon interactions on an equal footing, and establish the existence of novel physics which helps explain the unusually high superconducting transition temperatures in these systems. The Jahn-Teller phonons create a local (intramolecular) pairing that is surprisingly resistant to the Coulomb repulsion, despite the weakness of retardation in these low-bandwidth systems. The requirement for coherence throughout the solid to establish superconductivity then yields a very strong doping dependence to Tc, one consistent with experiment and much stronger than expected from standard Eliashberg theory.",0208454v1 2003-08-13,Physical properties of single-crystalline fibers of the colossal-magnetoresistance manganite La0.7Ca0.3MnO3,"We have grown high-quality single crystals of the colossal-magnetoresistance (CMR) material La0.7Ca0.3MnO3 by using the laser heated pedestal growth (LHPG) method. Samples were grown as fibers of different diameters, and with lengths of the order of centimeters. Their composition and structure were verified through X-ray diffraction, scanning electron microcopy with EDX (Energy Dispersive X-ray Analysis) and by Rietveld analysis. The quality of the crystalline fibers was confirmed by Laue and EBSD (Electron Backscatter Diffraction) patterns. Rocking curves performed along the fiber axis revealed a half-height width of 0.073 degrees. The CMR behavior was confirmed by electrical resistivity and magnetization measurements as a function of temperature.",0308245v1 2004-07-22,Real Space Imaging of the Microscopic Origins of the Ultrahigh Dielectric Constant in Polycrystalline CaCu3Ti4O12,"The origins of an ultrahigh dielectric constant in polycrystalline CaCu3Ti4O12 (CCTO) was studied using the combination of impedance spectroscopy, electron microscopy, and scanning probe microscopy (SPM). Impedance spectra indicate that the transport properties in the 0.1 Hz .. 1 MHz frequency range are dominated by a single parallel resistive-capacitive (RC) element with a characteristic relaxation frequency of 16 Hz. Dc potential distributions measurements by SPM illustrate that significant potential drops occur at the grain boundaries, which thus can be unambiguously identified as the dominant RC element. High frequency ac amplitude and phase distributions illustrate very weak contrast at the interfaces, which is indicative of strong capacitive coupling. These results demonstrate that the ultrahigh dielectric constant reported for polycrystalline CCTO materials are related to the grain boundary behavior.",0407608v1 2004-07-28,Room temperature tunneling magnetoresistance in magnetite based junctions: Influence of tunneling barrier,"Magnetite (Fe3O4) based tunnel junctions with turret/mesa structure have been investigated for different barrier materials (SrTiO3, NdGaO3, MgO, SiO2, and Al2O(3-x)). Junctions with a Ni counter electrode and an aluminium oxide barrier showed reproducibly a tunneling magnetoresistance (TMR) effect at room temperature of up to 5% with almost ideal switching behavior. This number only partially reflects the intrinsic high spin polarization of Fe3O4. It is considerably decreased due to an additional series resistance within the junction. Only SiO2 and Al2O(3-x) barriers provide magnetically decoupled electrodes as necessary for sharp switching. The observed decrease of the TMR effect as a function of increasing temperature is due to a decrease in spin polarization and an increase in spin-scattering in the barrier. Among the oxide half-metals magnetite has the potential to enhance the performance of TMR based devices.",0407725v1 2005-05-04,Tunable charge carriers and thermoelectricity of single-crystal Ba8Ga16Sn30,"We have grown single crystals of the type-VIII intermetallic clathrate Ba8Ga16Sn30 from both Sn and Ga flux, evaluated their compositions through electron microprobe analysis and studied their transport properties through measurements on temperature dependent resistivity, thermopower and Hall coefficient. Crystals grown in Sn flux show n-type carriers and those from Ga flux show p-type carriers, whereas all measured compositions remain very close to the stoichiometric 8:16:30 proportion of Ba:Ga:Sn, expected from charge-balance principles. Our results indicate a very high sensitivity of the charge carrier nature and density with respect to the growth conditions, leading to relevant differences in transport properties which point to the importance of tuning this material for optimal thermoelectric performance.",0505095v2 2005-05-14,"Surface morphology, structure and transport property of NaxCoO2 thin films grown by pulsed laser deposition","In this paper, we report the growth of NaxCoO2 thin films by pulsed-laser deposition (PLD). It is shown that the concentration of sodium is very sensitive to the substrate temperature and the target-substrate distance due to the evaporation of sodium during the deposition. alpha prime-phase Na0.75CoO2 and gamma- phase Na0.71CoO2 thin films can be obtained with different conditions. Correspondingly, the surface morphology of the films changes from flake-like to particle-like. The temperature dependence of resistivity for the films prepared with the optimal condition shows metallic behavior, consistent with the data of NaxCoO2 single crystals. This work demonstrates that PLD is a promising technique to get high quality NaxCoO2 thin films.",0505360v1 2005-10-19,Oxygen Isotope Effect on the Spin State Transition in (Pr$_{0.7}$Sm$_{0.3}$)$_{0.7}$Ca$_{0.3}$CoO${_3}$,"Oxygen isotope substitution is performed in the perovskite cobalt oxide (Pr$_{0.7}$Sm$_{0.3}$)$_{0.7}$Ca$_{0.3}$CoO${_3}$ which shows a sharp spin state transition from the intermediate spin (IS) state to the low spin (LS) state at a certain temperature. The transition temperature of the spin state up-shifts with the substitution of $^{16}O$ by $^{18}$O from the resistivity and magnetic susceptibility measurements. The up-shift value is 6.8 K and an oxygen isotope exponent ($\alpha_S$) is about -0.8. The large oxygen isotope effect indicates strong electron-phonon coupling in this material. The substitution of $^{16}$O by $^{18}$O leads to a decrease in the frequency of phonon and an increase in the effective mass of electron ($m$$^\ast$), so that the bandwidth W is decreased and the energy difference between the different spin states is increased. This is the reason why the $T_s$ is shifted to high temperature with oxygen isotopic exchange.",0510499v1 2005-10-24,Combining half-metals and multiferroics into epitaxial heterostructures for spintronics,"We report on the growth of epitaxial bilayers of the La2/3Sr1/3MnO3 (LSMO) half-metallic ferromagnet and the BiFeO3 (BFO) multiferroic, on SrTiO3(001) by pulsed laser deposition. The growth mode of both layers is two-dimensional, which results in unit-cell smooth surfaces. We show that both materials keep their properties inside the heterostructures, i.e. the LSMO layer (11 nm thick) is ferromagnetic with a Curie temperature of ~330K, while the BFO films shows ferroelectricity down to very low thicknesses (5 nm). Conductive-tip atomic force microscope mappings of BFO/LSMO bilayers for different BFO thicknesses reveal a high and homogeneous resistive state for the BFO film that can thus be used as a ferroelectric tunnel barrier in tunnel junctions based on a half-metal.",0510625v1 2006-05-22,Dissipative Van der Waals interaction between a small particle and a metal surface,"We use a general theory of the fluctuating electromagnetic field to calculate the friction force acting on a small neutral particle, e.g., a physisorbed molecule, or a nanoscale object with arbitrary dispersive and absorptive dielectric properties, moving near a metal surface. We consider the dependence of the electromagnetic friction on the temperature $T$, the separation $d$, and discuss the role of screening, non-local and retardation effects. We find that for high resistivity materials, the dissipative van der Waals interaction can be an important mechanism of vibrational energy relaxation of physisorbed molecules, and friction for microscopic solids. Several controversial topics related to electromagnetic dissipative shear stress is considered. The problem of local heating of the surface by an STM tip is also briefly commented on.",0605525v1 1999-04-15,Comparative Energy Dependence of Proton and Pion Degradation in Diamond,"A comparative theoretical study of the damages produced by protons and pions, in the energy range 50 MeV - 50 GeV, in diamond, is presented. The concentration of primary defects (CPD) induced by hadron irradiation is used to describe material degradation. The CPD has very different behaviours for protons and pions: the proton degradation is important at low energies and is higher than the pion one in the whole energy range investigated, with the exception of the Delta33 resonance region, where a large maximum of the degradation exists for pions. In comparison with silicon, the most investigated and the most studied material for detectors, diamond theoretically proves to be one order of magnitude more resistant, both to proton and pion irradiation.",9904342v1 2008-10-06,Theory of the spontaneous buckling of doped graphene,"Graphene is a realization of an esoteric class of materials -- electronic crystalline membranes. We study the interplay between the free electrons and the two-dimensional crystal, and find that it induces a substantial effect on the elastic structure of the membrane. For the hole-doped membrane, in particular, we predict a spontaneous buckling. In addition, attenuation of elastic waves is expected, due to the effect of corrugations on the bulk modulus. These discoveries have a considerable magnitude in graphene, affecting both its mesoscopic structure, and its electrical resistivity, which has an inherent asymmetry between hole- and electron-doped graphene.",0810.1062v4 2009-06-12,Giant magnetic anisotropy changes in Sr2CrReO6 thin films on BaTiO3,"The integration of ferromagnetic and ferroelectric materials into hybrid heterostructures yields multifunctional systems with improved or novel functionality. We here report on the structural, electronic and magnetic properties of the ferromagnetic double perovskite Sr2CrReO6, grown as epitaxial thin film onto ferroelectric BaTiO3. As a function of temperature, the crystal-structure of BaTiO3 undergoes phase transitions, which induce qualitative changes in the magnetic anisotropy of the ferromagnet. We observe abrupt changes in the coercive field of up to 1.2T along with resistance changes of up to 6.5%. These results are attributed to the high sensitivity of the double perovskites to mechanical deformation.",0906.2276v1 2010-01-22,Conducting interfaces between band insulating oxides: the LaGaO3/SrTiO3,"We show that the growth of the heterostructure LaGaO3/SrTiO3 yields the formation of a highly conductive interface. Our samples were carefully analyzed by high resolution electron microscopy, in order to assess their crystal perfection and to evaluate the abruptness of the interface. Their carrier density and sheet resistance are compared to the case of LaAlO3/SrTiO3 and a superconducting transition is found. The results open the route to widening the field of polar-non polar interfaces, pose some phenomenological constrains to their underlying physics and highlight the chance of tailoring their properties for future applications by adopting suitable polar materials.",1001.3956v2 2010-06-15,Fluorographene: Two Dimensional Counterpart of Teflon,"We report a stoichiometric derivative of graphene with a fluorine atom attached to each carbon. Raman, optical, structural, micromechanical and transport studies show that the material is qualitatively different from the known graphene-based nonstoichiometric derivatives. Fluorographene is a high-quality insulator (resistivity >10^12 Ohm per square) with an optical gap of 3 eV. It inherits the mechanical strength of graphene, exhibiting Young's modulus of 100 N/m and sustaining strains of 15%. Fluorographene is inert and stable up to 400C even in air, similar to Teflon.",1006.3016v2 2010-10-26,Graphene to Graphane: Novel Electrochemical Conversion,"A novel electrochemical means to generate atomic hydrogen, simplifying the synthesis and controllability of graphane formation on graphene is presented. High quality, vacuum grown epitaxial graphene (EG) was used as starting material for graphane conversion. A home-built electrochemical cell with Pt wire and exposed graphene as the anode and cathode, respectively, was used to attract H+ ions to react with the exposed graphene. Cyclic voltammetry of the cell revealed the potential of the conversion reaction as well as oxidation and reduction peaks, suggesting the possibility of electrochemically reversible hydrogenation. A sharp increase in D peak in the Raman spectra of EG, increase of D/G ratio, introduction of a peak at ~2930 cm-1 and respective peak shifts as well as a sharp increase in resistance showed the successful hydrogenation of EG. This conversion was distinguished from lattice damage by thermal reversal back to graphene at 1000{\deg}C.",1010.5458v1 2010-11-15,Transfer Printing Approach to All-Carbon Nanoelectronics,"Transfer printing methods are used to pattern and assemble monolithic carbon nanotube (CNT) thin-film transistors on large-area transparent, flexible substrates. Airbrushed CNT thin-films with sheet resistance 1kOhmsquare^{-1} at 80% transparency were used as electrodes, and high quality chemical vapor deposition (CVD)-grown CNT networks were used as the semiconductor component. Transfer printing was used to pre-pattern and assemble thin film transistors on polyethylene terephthalate (PET) substrates which incorporated Al_{2}O_{3}/poly-methylmethacrylate (PMMA) dielectric bi-layer. CNT-based ambipolar devices exhibit field-effect mobility in range 1 - 33 cm^{2}/Vs and on/off ratio ~10^{3}, comparable to the control devices fabricated using Au as the electrode material.",1011.3269v1 2011-07-05,Hidden spin liquid in an antiferromagnet: Applications to FeCrAs,"The recently studied material FeCrAs exhibits a surprising combination of experimental signatures, with metallic, Fermi liquid like specific heat but resistivity showing strong non-metallic character. The Cr sublattice posseses local magnetic moments, in the form of stacked (distorted) Kagome lattices. Despite the high degree of magnetic frustration, anti-ferromagnetic order develops below ~125K suggesting the non-magnetic Fe sublattice may play a role in stabilizing the ordering. From the material properties we propose a microscopic Hamiltonian for the low energy degrees of freedom, including the non-magnetic Fe sublattice, and study its properties using slave-rotor mean field theory. Using this approach we find a spin liquid phase on the Fe sublattice, which survives even in the presence of the magnetic Cr sublattice. Finally, we suggest that the features of FeCrAs can be qualitatively explained by critical fluctuations in the non-magnetic sublattice Fe due to proximity to a metal-insulator transition.",1107.1002v1 2011-11-16,Infrared Spectroscopy of Wafer-Scale Graphene,"We report on spectroscopy results from the mid- to far-infrared on wafer-scale graphene, grown either epitaxially on silicon carbide, or by chemical vapor deposition. The free carrier absorption (Drude peak) is simultaneously obtained with the universal optical conductivity (due to interband transitions), and the wavelength at which Pauli blocking occurs due to band filling. From these the graphene layer number, doping level, sheet resistivity, carrier mobility, and scattering rate can be inferred. The mid-IR absorption of epitaxial two-layer graphene shows a less pronounced peak at 0.37\pm0.02 eV compared to that in exfoliated bilayer graphene. In heavily chemically-doped single layer graphene, a record high transmission reduction due to free carriers approaching 40% at 250 \mum (40 cm-1) is measured in this atomically thin material, supporting the great potential of graphene in far-infrared and terahertz optoelectronics.",1111.3714v1 2011-12-22,Single crystal growth of YbRh2Si2 and YbIr2Si2,"We report on the single crystal growth of the heavy-fermion compounds YbRh2Si2 and YbIr2Si2 using a high-temperature indium-flux technique. The optimization of the initial composition and the temperature-time profile lead to large (up to 100 mg) and clean (\rho_0=0.5 \mu\Omega cm) single crystals of YbRh2Si2. Low-temperature resistivity measurements revealed a sample dependent temperature exponent below 10 K, which for the samples with highest quality deviates from a linear-in-T behaviour. Furthermore, we grew single crystals of the alloy series Yb(Rh_(1-x)Ir_x)2Si2 with 0 50%, but fixed moisture-contents (i.e., basic creep), arises from a dissolution-precipitation mechanism, active at nanoscale grain contacts, as is often observed in a geological context, e.g., when rocks are exposed to sustained loads, in moist environments. Based on micro-indentation and vertical scanning interferometry experiments, and molecular dynamics simulations carried out on calcium-silicate-hydrates (C-S-H's), the major binding phase in concrete, of different compositions, we show that creep rates are well correlated to dissolution rates - an observation which supports the dissolution-precipitation mechanism as the origin of concrete creep. C-S-H compositions featuring high resistance to dissolution, and hence creep are identified - analysis of which, using topological constraint theory, indicates that these compositions present limited relaxation modes on account of their optimally connected (i.e., constrained) atomic networks.",1508.07082v1 2015-09-11,High thermoelectric performance and low thermal conductivity of densified LaOBiSSe,"In this study, we examined the thermoelectric properties of the layered bismuth-chalcogenide-based (BiCh2-based) compound LaOBiSSe, which is expected to be a new candidate material for thermoelectric applications. Densified samples were obtained with a hot-press method. The results of the X-ray diffraction measurements showed that the samples obtained were weakly oriented. This affected the resistivity (r) and Seebeck coefficient (S) of the samples because they are dependent upon the orientation of the crystal structure. The values obtained for the power factor (S2/r) when measured perpendicular to the pressing direction (P1) were higher than that when measured parallel to the pressing direction (P2). The thermal conductivity (k) of the samples was also sensitive to the orientation. The values of k measured along P2 were lower than that measured along P1. The highest figure-of-merit (approximately 0.36) was obtained at around 650 K in both directions, i.e., P1 and P2.",1509.03387v1 2016-04-22,Thermoelectric Properties of Antiperovskite Calcium Oxides Ca3PbO and Ca3SnO,"We report the thermoelectric properties of polycrystalline samples of Ca3Pb1-xBixO (x = 0, 0.1, 0.2) and Ca3SnO, both crystallizing in a cubic antiperovskite-type structure. The Ca3SnO sample shows metallic resistivity and its thermoelectric power approaches 100 uV K-1 at room temperature, resulting in the thermoelectric power factor of Ca3SnO being larger than that of Ca3Pb1-xBixO. On the basis of Hall and Sommerfeld coefficients, the Ca3SnO sample is found to be a p-type metal with a carrier density of ~1019 cm-3, a mobility of ~80 cm2 V-1 s-1, both comparable to those in degenerated semiconductors, and a moderately large hole carrier effective mass. The coexistence of moderately high mobility and large effective mass observed in Ca3SnO, as well as possible emergence of a mutivalley electronic structure with a small band gap at low-symmetry points in k-space, suggests that the antiperovskite Ca oxides have strong potential as a thermoelectric material.",1604.06541v2 2016-04-26,A Sinusoidally-Architected Helicoidal Biocomposite,"A fibrous herringbone-modified helicoidal architecture is identified within the exocuticle of an impact-resistant crustacean appendage. This previously unreported composite microstructure, which features highly textured apatite mineral templated by an alpha-chitin matrix, provides enhanced stress redistribution and energy absorption over the traditional helicoidal design under compressive loading. Nanoscale toughening mechanisms are also identified using high load nanoindentation and in-situ TEM picoindentation.",1604.07798v2 2016-05-04,Atomically Thin Boron Nitride: Unique Properties and Applications,"Atomically thin boron nitride (BN) is an important two-dimensional (2D) nanomaterial, with many properties distinct from graphene. In this feature article, these unique properties and associated applications often not possible from graphene are outlined. The article starts with characterization and identification of atomically thin BN. It is followed by demonstrating their strong oxidation resistance at high temperatures and applications in protecting metals from oxidation and corrosion. As flat insulators, BN nanosheets are ideal dielectric substrates for surface enhanced Raman spectroscopy (SERS) and electronic devices based on 2D heterostructures. The light emission of BN nanosheets in the deep ultraviolet (DUV) and ultraviolet (UV) regions are also included for its scientific and technological importance. The last part is dedicated to synthesis, characterization, and optical properties of BN nanoribbons, a special form of nanosheets.",1605.01136v1 2016-05-06,Superconducting gap structure of FeSe,"The microscopic mechanism governing the zero-resistance flow of current in some iron-based, high-temperature superconducting materials is not well understood up to now. A central issue concerning the investigation of these materials is their superconducting gap symmetry and structure. Here we present a combined study of low-temperature specific heat and scanning tunnelling microscopy measurements on single crystalline FeSe. The results reveal the existence of at least two superconducting gaps which can be represented by a phenomenological two-band model. The analysis of the specific heat suggests significant anisotropy in the gap magnitude with deep gap minima. The tunneling spectra display an overall ""U""-shaped gap close to the Fermi level away as well as on top of twin boundaries. These results are compatible with the anisotropic nodeless models describing superconductivity in FeSe.",1605.01908v2 2016-05-24,Pressure-Induced Confined Metal from the Mott Insulator Sr3Ir2O7,"The spin-orbit Mott insulator Sr3Ir2O7 provides a fascinating playground to explore insulator-metal transition driven by intertwined charge, spin, and lattice degrees of freedom. Here, we report high pressure electric resistance and resonant inelastic x ray scattering measurements on single crystal Sr3Ir2O7 up to 63 65 GPa at 300 K. The material becomes a confined metal at 59.5 GPa, showing metallicity in the ab plane but an insulating behavior along the c axis. Such an unusual phenomenon resembles the strange metal phase in cuprate superconductors. Since there is no sign of the collapse of spin orbit or Coulomb interactions in x-ray measurements, this novel insulator metal transition is potentially driven by a first-order structural change at nearby pressures. Our discovery points to a new approach for synthesizing functional materials.",1605.07582v1 2016-11-08,Valley Hall Effect and Nonlocal Transport in Strained Graphene,"Graphene subject to high levels of shear strain leads to strong pseudo-magnetic fields resulting in the emergence of Landau levels. Here we show that, with modest levels of strain, graphene can also sustain a classical valley hall effect (VHE) that can be detected in nonlocal transport measurements. We provide a theory of the strain-induced VHE starting from the quantum Boltzmann equation. This allows us to show that, averaging over short-range impurity configurations destroys quantum coherence between valleys, leaving the elastic scattering time and inter-valley scattering rate as the only parameters characterizing the transport theory. Using the theory, we compute the nonlocal resistance of a Hall bar device in the diffusive regime. Our theory is also relevant for the study of moderate strain effects in the (nonlocal) transport properties of other two-dimensional materials and van der Walls heterostructures.",1611.02382v2 2016-11-11,Microfluidization of graphite and formulation of graphene-based conductive inks,"We report the exfoliation of graphite in aqueous solutions under high shear rate [$\sim10^8s^{-1}$] turbulent flow conditions, with a 100\% exfoliation yield. The material is stabilized without centrifugation at concentrations up to 100 g/L using carboxymethylcellulose sodium salt to formulate conductive printable inks. The sheet resistance of blade coated films is below$\sim2\Omega/\square$. This is a simple and scalable production route for graphene-based conductive inks for large area printing in flexible electronics.",1611.04467v1 2016-12-26,Observation of quantum oscillations in FIB fabricated nanowires of topological insulator (Bi2Se3),"Since last few years, research based on topological insulators (TI) is in great interests due to intrinsic exotic fundamental properties and future potential applications such as quantum computers or spintronics. The fabrication of TI nanodevices and study on their transport properties mostly focused on high quality crystalline nanowires or nanoribbons. Here we report robust approach of Bi2Se3 nanowire formation from deposited flakes using ion beam milling method. The fabricated Bi2Se3 nanowire devices have been employed to investigate the robustness of topological surface state (TSS) to gallium ion doping and any deformation in the material due to fabrication tools. We report the quantum oscillations in magnetoresistance curves under the parallel magnetic field. The resistance versus magnetic field curves have been studied and compared with Aharonov-Bohm (AB) interference effects which further demonstrate the transport through TSS. The fabrication route and observed electronic transport properties indicate clear quantum oscillations and can be exploited further in studying the exotic electronic properties associated with TI based nanodevices.",1612.08353v1 2017-09-26,SnAs-based layered superconductor NaSn2As2,"Superconductivity with exotic properties has often been discovered in materials with a layered (two-dimensional) crystal structure. The low dimensionality affects the electronic structure of materials, which could realize a high transition temperature (Tc) and/or unconventional pairing mechanisms. Here, we report the superconductivity in a layered tin arsenide NaSn2As2. The crystal structure consists of (Sn2As2)2- bilayers, which is bound by van-der-Waals forces, separated by Na+ ions. Measurements of electrical resistivity and specific heat confirm the bulk nature of superconductivity of NaSn2As2 with Tc of 1.3 K. Our results propose that the SnAs layers will be a basic structure providing another universality class of a layered superconducting family, and it provides a new platform for the physics and chemistry of low-dimensional superconductors with lone pair electrons.",1709.08899v2 2017-11-10,Giant anisotropic magnetoresistance and planar Hall effect in the Dirac semimetal Cd3As2,"Anisotropic magnetoresistance is the change tendency of resistance of a material on the mutual orientation of the electric current and the external magnetic field. Here, we report experimental observations in the Dirac semimetal Cd3As2 of giant anisotropic magnetoresistance and its transverse version, called the planar Hall effect. The relative anisotropic magnetoresistance is negative and up to -68% at 2 K and 10 T. The high anisotropy and the minus sign in this isotropic and nonmagnetic material are attributed to a field-dependent current along the magnetic field, which may be induced by the Berry curvature of the band structure. This observation not only reveals unusual physical phenomena in Weyl and Dirac semimetals, but also finds additional transport signatures of Weyl and Dirac fermions other than negative magnetoresistance.",1711.03671v2 2017-11-15,Revisiting the electron-doped SmFeAsO: enhanced superconductivity up to 58.6 K by Th and F codoping,"In the iron-based high-Tc bulk superconductors, Tc above 50K was only observed in the electron-doped 1111-type compounds. Here we revisit the electron-doped SmFeAsO polycrystals to make a further investigation for the highest T-c in these materials. To introduce more electron carriers and less crystal lattice distortions, we study the Th and F codoping effects into the Sm-O layers with heavy electron doping. Dozens of Sm1-x Th-x FeAsO1-y F-y samples are synthesized through the solid state reaction method, and these samples are carefully characterized by the structural, resistive, and magnetic measurements. We find that the codoping of Th and F clearly enhances the superconducting T-c more than the Th or F single-doped samples, with the highest record T-c up to 58.6K when x= 0.2 and y= 0.225. Further element doping causes more impurities and lattice distortions in the samples with a weakened superconductivity.",1711.05440v1 2018-01-19,Observation of Meissner effect in potassium-doped \emph{p}-quinquephenyl},"The chain-like organic compounds with conjugated structure have the potential to become high temperature superconductors. We examine this idea by choosing p-quinquephenyl with five phenyl rings connected in para position. The dc magnetic susceptibility measurements provide solid evidence for the presence of Meissner effect when the compound is doped by potassium. The real part of the ac susceptibility shows exactly same transition temperature as that in dc magnetization, and the imaginary part of nearly zero value after transition implies the realization of zero-resistivity. All these features support the existence of superconductivity with a critical temperature of 7.3 K in this material. The occurrence of bipolarons revealed by Raman spectra guarantees potassium metal intercalated into p-quinquephenyl and suggests the important role of this elementary excitation played on superconductivity.",1801.06324v2 2018-01-19,Pressure-induced superconductivity in palladium sulfide,"An extended study on PdS is carried out with the measurements of the resistivity, Hall coefficient, Raman scattering, and X-ray diffraction at high pressures up to 42.3 GPa. With increasing pressure, superconductivity is observed accompanying with a structural phase transition at around 19.5 GPa. The coexistence of semiconducting and metallic phases observed at normal state is examined by the Raman scattering and X-ray diffraction between 19.5 and 29.5 GPa. After that, only the metallic normal state maintains with an almost constant superconducting transition temperature. The similar evolution between the superconducting transition temperature and carrier concentration with pressure supports the phonon-mediated superconductivity in this material. These results highlight the important role of pressure played in inducing superconductivity from these narrow band-gap semiconductors.",1801.06330v1 2018-02-07,"Structure, magnetic and transport properties of epitaxial thin films of equiatomic CoFeMnGe quaternary Heusler alloy","Future spintronics requires the realization of thin film of half-metallic ferromagnets having high Curie temperature and 100\% spin polarization at the Fermi level for potential spintronics applications. In this paper, we report the epitaxial thin films growth of half-metallic CoFeMnGe Heusler alloy on MgO (001) substrate using pulsed laser deposition system, along with the study of structural, magnetic and transport properties. The magnetic property measurements of the thin film suggest a soft ferromagnetic state at room temperature with an in-plane magnetic anisotropy and a Curie temperature well above the room temperature. Anisotropic magnetoresistance (AMR) ratio and temperature dependent electrical resistivity measurements of the thin film indicate the compound to be half-metallic in nature and therefore suitable for the fabrications of spintronics devices.",1802.02413v1 2018-03-12,Sub 20 meV Schottky barriers in metal/MoTe2 junctions,"The newly emerging class of atomically-thin materials has shown a high potential for the realisation of novel electronic and optoelectronic components. Amongst this family, semiconducting transition metal dichalcogenides (TMDCs) are of particular interest. While their band gaps are compatible with those of conventional solid state devices, they present a wide range of exciting new properties that is bound to become a crucial ingredient in the future of electronics. To utilise these properties for the prospect of electronics in general, and long-wavelength-based photodetectors in particular, the Schottky barriers formed upon contact with a metal and the contact resistance that arises at these interfaces have to be measured and controlled. We present experimental evidence for the formation of Schottky barriers as low as 10 meV between MoTe2 and metal electrodes. By varying the electrode work functions, we demonstrate that Fermi level pinning due to metal induced gap states at the interfaces occurs at 0.14 eV above the valence band maximum. In this configuration, thermionic emission is observed for the first time at temperatures between 40 K and 75 K. Finally, we discuss the ability to tune the barrier height using a gate electrode.",1803.04164v1 2018-04-09,Dislocation-induced thermal transport anisotropy in single-crystal group-III nitride films,"Dislocations, one-dimensional lattice imperfections, are common to technologically important materials such as III-V semiconductors, and adversely affect heat dissipation in e.g., nitride-based high-power electronic devices. For decades, conventional models based on nonlinear elasticity theory have predicted this thermal resistance is only appreciable when heat flux is perpendicular to the dislocations. However, this dislocation-induced anisotropic thermal transport has yet to be seen experimentally. In this study, we measure strong thermal transport anisotropy governed by highly oriented threading dislocation arrays along the cross-plane direction in micron-thick, single-crystal indium nitride (InN) films. We find that the cross-plane thermal conductivity is more than tenfold higher than the in-plane thermal conductivity at 80 K when the dislocation density is on the order of ~3x10^10 cm^-2. This large anisotropy is not predicted by the conventional models. With enhanced understanding of dislocation-phonon interactions, our results open new regimes for tailoring anisotropic thermal transport with line defects, and will facilitate novel methods for directed heat dissipation in thermal management of diverse device applications.",1804.02825v1 2018-05-01,Strongly correlated proton-doped perovskite nickelate memory devices,"We demonstrate memory devices based on proton doping and re-distribution in perovskite nickelates (RNiO3, {R=Sm,Nd}) that undergo filling-controlled Mott transition. Switching speeds as high as 30 ns in two-terminal devices patterned by electron-beam lithography is observed. The state switching speed reported here are 300X greater than what has been noted with proton-driven resistance switching to date. The ionic-electronic correlated oxide memory devices also exhibit multi-state non-volatile switching. The results are of relevance to use of quantum materials in emerging memory and neuromorphic computing.",1805.00527v1 2018-06-21,Strange metallicity in the doped Hubbard model,"Strange or bad metallic transport, defined by its incompatibility with conventional quasiparticle pictures, is a theme common to strongly correlated materials and ubiquitous in many high temperature superconductors. The Hubbard model represents a minimal starting point for modeling strongly correlated systems. Here we demonstrate strange metallic transport in the doped two-dimensional Hubbard model using determinantal quantum Monte Carlo calculations. Over a wide range of doping, we observe resistivities exceeding the Mott-Ioffe-Regel limit with linear temperature dependence. The temperatures of our calculations extend to as low as 1/40 the non-interacting bandwidth, placing our findings in the degenerate regime relevant to experimental observations of strange metallicity. Our results provide a foundation for connecting theories of strange metals to models of strongly correlated materials.",1806.08346v2 2018-09-13,Superconductivity in LaPd2Bi2 with CaBe2Ge2-type structure,"Here we report the synthesis and superconductivity of a novel ternary compound LaPd2Bi2. Shiny plate-like single crystals of LaPd2Bi2 were first synthesized by high-temperature solution method with PdBi flux. X-ray diffraction analysis indicates that LaPd2Bi2 belongs to the primitive tetragonal CaBe2Ge2-type structure with the space group P4/nmm (No. 129), and the refined lattice parameters are a = 4.717(2) {\AA}, c = 9.957(3) {\AA}. Electrical resistivity and magnetic susceptibility measurements reveal that LaPd2Bi2 undergoes a superconducting transition at 2.83 K and exhibits the characteristics of type-II superconductivity. The discovery of superconductivity in LaPd2Bi2 with CaBe2Ge2-type structure may help to further understand the possible relationship between the occurrence of superconductivity and the crystal structures in 122-type materials.",1809.04811v1 2019-05-08,Miniature Multi-Level Optical Memristive Switch Using Phase Change Material,"The optical memristive switches are electrically activated optical switches that can memorize the current state. They can be used as optical latching switches in which the switching state is changed only by applying an electrical Write/Erase pulse and maintained without external power supply. We demonstrate an optical memristive switch based on a silicon MMI structure covered with nanoscale-size Ge2Sb2Te5 (GST) material on top. The phase change of GST is triggered by resistive heating of the silicon layer beneath GST with an electrical pulse. Experimental results reveal that the optical transmissivity can be tuned in a controllable and repeatable manner with the maximum transmission contrast exceeding 20 dB. Partial crystallization of GST is obtained by controlling the width and amplitude of the electric pulses. Crucially, we also demonstrate that both Erase and Write operations, to and from any intermediate level, are possible with accurate control of the electrical pulses. Our work marks a significant step forward towards realizing photonic memristive switches without static power consumption, which are highly demanded in high-density large-scale integrated photonics.",1905.03163v1 2020-03-02,Structural and Magnetic Properties of Molecular Beam Epitaxy Grown Chromium Selenide Thin Films,"Chromium selenide thin films were grown epitaxially on Al${_2}$O${_3}$(0001) and Si(111)-(7${\times}$7) substrates using molecular beam epitaxy (MBE). Sharp streaks in reflection high-energy electron diffraction and triangular structures in scanning tunneling microscopy indicate a flat smooth film growth along the c-axis, and is very similar to that from a hexagonal surface. X-ray diffraction pattern confirms the growth along the c-axis with c-axis lattice constant of 17.39 {\AA}. The grown film is semiconducting, having a small band gap of about 0.034 eV, as calculated from the temperature dependent resistivity. Antiferromagnetic nature of the film with a N\'eel temperature of about 40 K is estimated from the magnetic exchange bias measurements. A larger out-of-plane exchange bias, along with a smaller in-plane exchange bias is observed below 40 K. Exchange bias training effects are analyzed based on different models and are observed to be following a modified power-law decay behavior.",2003.01199v1 2017-03-01,Chemical and Lattice Stability of the Tin Sulfides,"The tin sulfides represent a materials platform for earth-abundant semiconductor technologies. We present a first-principles study of the five known and proposed phases of SnS together with SnS2 and Sn2S3. Lattice-dynamics techniques are used to evaluate the dynamical stability and temperature-dependent thermodynamic free energy, and we also consider the effect of dispersion forces on the energetics. The recently identified {\pi}-cubic phase of SnS is found to be metastable with respect to the well-known orthorhombic Pnma/Cmcm equilibrium. The Cmcm phase is a low-lying saddle point between Pnma minima on the potential-energy surface, and is observed as an average structure at high temperatures. Bulk rocksalt and zincblende phases are found to be dynamically unstable, and we show that whereas rocksalt SnS can potentially be stabilised under a reduction of the lattice constant, the hypothetical zincblende phase proposed in several earlier studies is extremely unlikely to form. We also investigate the stability of Sn2S3 with respect to SnS and SnS2, and find that both dispersion forces and vibrational contributions to the free energy are required to explain its experimentally-observed resistance to decomposition.",1703.00361v2 2017-03-11,Sign reversal of magnetoresistance and p to n transition in Ni doped ZnO thin film,"We report the magnetoresistance and nonlinear Hall effect studies over a wide temperature range in pulsed laser deposited Ni0.07Zn0.93O thin film. Negative and positive contributions to magnetoresistance at high and low temperatures have been successfully modeled by the localized magnetic moment and two band conduction process involving heavy and light hole subbands, respectively. Nonlinearity in the Hall resistance also agrees well with the two channel conduction model. A negative Hall voltage has been found for T $\gte 50 K$, implying a dominant conduction mainly by electrons whereas positive Hall voltage for T less than 50 K shows hole dominated conduction in this material. Crossover in the sign of magnetoresistance from negative to positive reveals the spin polarization of the charge carriers and hence the applicability of Ni doped ZnO thin film for spintronic applications.",1703.03942v1 2018-10-01,Quantum transport in a compensated semimetal W2As3 with nontrivial Z2 indices,"We report a topological semimetal W2As3 with a space group C2/m. Based on the first-principles calculations, band crossings are partially gapped when spin-orbit coupling is included. The Z2 indices at the electron filling are [1;111], characterizing a strong topological insulator and topological surface states. From the magnetotransport measurements, nearly quadratic field dependence of magnetoresistance (MR) (B || [200]) at 3 K indicates an electron-hole compensated compound whose longitudinal MR reaches 115 at 3 K and 15 T. In addition, multiband features are detected from the high-magnetic-field Shubnikov-de Haas (SdH) oscillation, Hall resistivity, and band calculations. A nontrivial pi Berry's phase is obtained, suggesting the topological feature of this material. A two- band model can fit well the conductivity and Hall coefficient. Our experiments manifest that the transport properties of W2As3 are in good agreement with the theoretical calculations.",1810.00665v1 2019-07-05,Giant enhancement of Piezo-resistance in ballistic graphene due to transverse electric fields,"We investigate the longitudinal and transverse piezoresistance effect in suspended graphene in the ballistic regime. Utilizing parametrized tight binding Hamiltonian from ab initio calculations along with Landauer quantum transport formalism, we devise a methodology to evaluate the piezoresistance effect in 2D materials especially in graphene. We evaluate the longitudinal and transverse gauge factor of graphene along armchair and zigzag directions in the linear elastic limit ($0\%$-$10\%$). The longitudinal and transverse gauge factors are identical along armchair and zigzag directions. Our model predicts a significant variation ($\approx 1000\% $ change) in transverse gauge factor compared to longitudinal gauge factor along with sign inversion. The calculated value of longitudinal gauge factor is $\approx 0.3$ whereas the transverse gauge factor is $\approx -3.3$. We rationalize our prediction using deformation of Dirac cone and change in separation between transverse modes due to longitudinal and transverse strain, leading to an inverse change in gauge factor. The results obtained herein may serve as a template for high strain piezoresistance effect of graphene in nano electromechanical systems.",1907.02896v1 2020-04-23,Experimental evidence of monolayer AlB$_2$ with symmetry-protected Dirac cones,"Monolayer AlB$_2$ is composed of two atomic layers: honeycomb borophene and triangular aluminum. In contrast with the bulk phase, monolayer AlB$_2$ is predicted to be a superconductor with a high critical temperature. Here, we demonstrate that monolayer AlB$_2$ can be synthesized on Al(111) via molecular beam epitaxy. Our theoretical calculations revealed that the monolayer AlB$_2$ hosts several Dirac cones along the $\Gamma$--M and $\Gamma$--K directions; these Dirac cones are protected by crystal symmetries and are thus resistant to external perturbations. The extraordinary electronic structure of the monolayer AlB$_2$ was confirmed via angle-resolved photoemission spectroscopy measurements. These results are likely to stimulate further research interest to explore the exotic properties arising from the interplay of Dirac fermions and superconductivity in two-dimensional materials.",2004.10916v1 2020-09-13,Extreme softness of brain matter in simple shear,"We show that porcine brain matter can be modelled accurately as a very soft rubber-like material using the Mooney-Rivlin strain energy function, up to strains as high as 60\%. This result followed from simple shear experiments performed on small rectangular fresh samples ($2.5$ cm$^3$ and $1.1$ cm$^3$) at quasi-static strain rates. They revealed a linear shear stress--shear strain relationship ($R^2> 0.97 $), characteristic of Mooney-Rivlin materials at large strains. We found that porcine brain matter is about 30 times less resistant to shear forces than a silicone gel. We also verified experimentally that brain matter exhibits the positive Poynting effect of nonlinear elasticity, and numerically that the stress and strain fields remain mostly homogeneous throughout the thickness of the samples in simple shear.",2009.06102v1 2020-09-29,Dimensional Crossover Tuned by Pressure in Layered Magnetic NiPS3,"Layered magnetic transition-metal thiophosphate NiPS3 has unique two-dimensional (2D) magnetic properties and electronic behavior. The electronic band structure and corresponding magnetic state are expected to sensitive to the interlayer interaction, which can be tuned by external pressure. Here, we report an insulator-metal transition accompanied with magnetism collapse during the 2D-3D crossover in structure induced by hydrostatic pressure. A two-stage phase transition from monoclinic (C2=m) to trigonal (P-31m) lattice is identified by ab initio simulation and confirmed by high-pressure XRD and Raman data, corresponding to a layer by layer slip mechanism along the a-axis. Temperature dependence resistance measurements and room temperature infrared spectroscopy show that the insulator-metal transition occurs near 20 GPa as well as magnetism collapse, which is further confirmed by low temperature Raman measurement and theoretical calculation. These results establish a strong correlation among the structural change, electric transport, and magnetic phase transition and expand our understandings about the layered magnetic materials.",2009.14051v1 2022-02-23,The honeycomb and hyperhoneycomb polymorphs of IrI$_3$,"The synthesis of IrI$_3$ at high pressure in its layered honeycomb polymorph is reported. Its crystal structure is refined by single crystal X-ray diffraction. Faults in the honeycomb layer stacking are observed by single crystal diffraction, synchrotron powder diffraction, and transmission electron microscopy. A previously unreported hyperhoneycomb polymorph of IrI$_3$ ($\beta$-IrI$_3$), is also described. Its structure in space group Fddd is determined by single crystal XRD. Both materials are highly-resistive diamagnetic semiconductors, consistent with a low spin d$^6$ configuration for Ir(III). The two- and three-dimensional Ir arrays in these polymorphs of IrI$_3$ are analogous to those found in the $\alpha$- and $\beta$- polymorphs of Li$_2$IrO$_3$, although the Ir electron configurations are different.",2202.11658v1 2014-01-10,Ferroelectric-like SrTiO3 surface dipoles probed by graphene,"The electrical transport properties of graphene are greatly influenced by its environment. Owing to its high dielectric constant, strontium titanate (STO) is expected to suppress the long-range charged impurity scattering and consequently to enhance the mobility. However, the absence of such enhancement has caused some controversies regarding the scattering mechanism. In graphene devices transferred from SiO2 to STO using a newly developed technique, we observe a moderate mobility enhancement near the Dirac point, which is the point of charge neutrality achieved by adjusting the Fermi level. While bulk STO is not known as a ferroelectric material, its surface was previously reported to exhibit an outward displacement of oxygen atoms and ferroelectric-like dipole moment. When placed on STO, graphene shows strong and asymmetric hysteresis in resistivity, which is consistent with the dipole picture associated with the oxygen displacement. The hysteretic response of the surface dipole moment diminishes the polarizability, therefore weakens the ability of STO to screen the Coulomb potential of the impurities.",1401.2222v1 2017-05-01,Large Thermoelectric Power Factor at Low Temperatures in One-Dimensional Telluride Ta4SiTe4,"We report the discovery of a very large thermoelectric power over -400 microV K-1 in the whisker crystals of a one-dimensional telluride Ta4SiTe4, while maintaining a low electrical resistivity of rho = 2 mohm cm, yielding a very large power factor of P = 80 microW cm-1 K-2 at an optimum temperature of 130 K. This temperature is widely controlled from the cryogenic temperature of 50 K to room temperature by chemical doping, resulting in the largest P of 170 microW cm-1 K-2 at 220-280 K. These P values far exceed those of the Bi2Te3-Sb2Te3 alloys at around room temperature, offering an avenue for realizing the practical-level thermoelectric cooling at low temperatures. The coexistence of a one-dimensional electronic structure and a very small band gap appearing in the vicinity of the Dirac semimetals probably causes the very large power factors in Ta4SiTe4, indicating that the ""one-dimensional Dirac semimetal"" is a promising way to find high-performance thermoelectric materials for the low temperature applications.",1705.00404v1 2017-08-25,Spin torque control of antiferromagnetic moments in NiO,"For a long time, there have been no efficient ways of controlling antiferromagnets. Quite a strong magnetic field was required to manipulate the magnetic moments because of a high molecular field and a small magnetic susceptibility. It was also difficult to detect the orientation of the magnetic moments since the net magnetic moment is effectively zero. For these reasons, research on antiferromagnets has not been progressed as drastically as that on ferromagnets which are the main materials in modern spintronic devices. Here we show that the magnetic moments in NiO, a typical natural antiferromagnet, can indeed be controlled by the spin torque with a relatively small electric current density (~5 x 10^7 A/cm^2) and their orientation is detected by the transverse resistance resulting from the spin Hall magnetoresistance . The demonstrated techniques of controlling and detecting antiferromagnets would outstandingly promote the methodologies in the recently emerged ""antiferromagnetic spintronics"". Furthermore, our results essentially lead to a spin torque antiferromagnetic memory.",1708.07682v1 2019-03-13,"Hydrodynamic Phonon Transport: Past, Present, and Prospect","The hydrodynamic phonon transport was studied several decades ago for verifying the quantum theory of lattice thermal transport. Recent prediction of significant hydrodynamic phonon transport in graphitic materials shows its practical importance for high thermal conductivity materials and brought a renewed attention. As the study on this topic has been inactive to some extent for several decades, we aim at providing a brief overview of the past studies as well as very recent studies. The topics we discuss in this chapter include the collective motion of phonons, several approaches to solve the Peierls-Boltzmann transport equation for hydrodynamic phonon transport, the role of normal scattering for thermal resistance, and the propagation of second sound. Then, we close this chapter with our perspectives for the future studies and the practical implication of hydrodynamic phonon transport.",1903.05731v1 2019-04-12,Synthesis of anti-perovskite-type carbides and nitrides from metal oxides and melamine,"Four anti-perovskite-type compounds, ZnNNi3, ZnCNi3, SnNCo3, and SnCCo3, are synthesised through reactions between ingredient metal oxides and organic compound melamine (C3H6N6). ZnNNi3 and ZnCNi3 are selectively synthesised by choosing different reaction temperatures and nominal oxide-to-melamine ratios. SnNCo3 is synthesised for the first time by this melamine method. Resistivity, magnetisation, and heat capacity measurements reveal that SnNCo3 is a correlated metal with a high density of states at the Fermi level. Our results demonstrate that this feasible synthetic route using melamine is useful in the search for complex metal carbides and nitrides toward novel functional materials.",1904.06103v1 2019-12-23,Hydride Vapor-Phase Epitaxy Reactor for Bulk GaN Growth,"An HVPE reactor for the growth of bulk GaN crystals with a diameter of 50 mm was developed. Growth rate non-uniformity of 1% was achieved using an axisymmetric vertical gas injector with stagnation point flow. Chemically-resistant refractory materials were used instead of quartz in the reactor hot zone. High-capacity external gallium precursor sources were developed for the non-stop growth of the bulk GaN layers. A load-lock vacuum chamber and a dry in-situ growth chamber cleaning were implemented to improve the growth process reproducibility. Freestanding GaN crystals with a diameter of 50 mm were grown with the reactor.",1912.11010v1 2012-03-27,Shadow evaporation of epitaxial Al/Al2O3/Al tunnel junctions on sapphire utilizing an inorganic bilayer mask,"This letter describes a new inorganic shadow mask that has been employed for the evaporation of all-epitaxial Al/Al2O3/Al superconducting tunnel junctions. Organic resists that are commonly used for shadow masks and other lift-off processes are not compatible with ultra-high vacuum deposition systems, and they can break down at even moderately elevated temperatures. The inorganic mask described herein does not suffer these same shortcomings. It was fabricated from a Ge/Nb bilayer, comprising suspended Nb bridges supported by an undercut Ge sacrificial layer. Utilizing such a bilayer mask on C-plane sapphire, the growth of epitaxial Al tunnel junctions was achieved using molecular beam epitaxy. Crystalline Al2O3 was grown diffusively at 300 C in a molecular oxygen background of 2.0 utorr, while amorphous oxide was grown at room temperature and 25 mtorr. A variety of analysis techniques were employed to evaluate the materials, and tunnel junction current-voltage characteristics were measured at millikelvin temperatures.",1203.6007v1 2012-06-14,Conduction in jammed systems of tetrahedra,"Control of transport processes in composite microstructures is critical to the development of high performance functional materials for a variety of energy storage applications. The fundamental process of conduction and its control through the manipulation of granular composite attributes (e.g., grain shape) are the subject of this work. We show that athermally jammed packings of tetrahedra with ultra-short range order exhibit fundamentally different pathways for conduction than those in dense sphere packings. Highly resistive granular constrictions and few face-face contacts between grains result in short-range distortions from the mean temperature field. As a consequence, 'granular' or differential effective medium theory predicts the conductivity of this media within 10% at the jamming point; in contrast, strong enhancement of transport near interparticle contacts in packed-sphere composites results in conductivity divergence at the jamming onset. The results are expected to be particularly relevant to the development of nanomaterials, where nanoparticle building blocks can exhibit a variety of faceted shapes.",1206.2990v1 2016-09-06,Effect of morphology and defectiveness of graphene-related materials on the electrical and thermal conductivity of their polymer nanocomposites,"In this work, electrically and thermally conductive poly (butylene terephthalate) nanocomposites were prepared by in-situ ring-opening polymerization of cyclic butylene terephthalate (CBT) in presence of a tin-based catalyst. One type of graphite nanoplatelets (GNP) and two different grades of reduced graphene oxide (rGO) were used. Furthermore, high temperature annealing treatment under vacuum at 1700{\deg}C was carried out on both RGO to reduce their defectiveness and study the correlation between the electrical/thermal properties of the nanocomposites and the nanoflakes structure/defectiveness. The morphology and quality of the nanomaterials were investigated by means of electron microscopy, x-ray photoelectron spectroscopy, thermogravimetry and Raman spectroscopy. Thermal, mechanical and electrical properties of the nanocomposites were investigated by means of rheology, dynamic mechanical thermal analysis, volumetric resistivity and thermal conductivity measurements. Physical properties of nanocomposites were correlated with the structure and defectiveness of nanoflakes, evidencing a strong dependence of properties on nanoflakes structure and defectiveness. In particular, a significant enhancement of both thermal and electrical conductivities was demonstrated upon the reduction of nanoflakes defectiveness.",1609.01581v2 2016-09-22,Crystal structure and low-energy Einstein mode in ErV$_2$Al$_{20}$ intermetallic cage compound,"Single crystals of a new ternary aluminide ErV$_2$Al$_{20}$ were grown using a self-flux method. The crystal structure was determined by powder X-ray diffraction measurements and Rietveld refinement, and physical properties were studied by means of electrical resistivity, magnetic susceptibility and specific heat measurements. These measurements reveal that ErV$_2$Al$_{20}$ is a Curie-Weiss paramagnet down to 1.95 K with an effective magnetic moment $\mu_{eff}$ = 9.27(1) $\mu_B$ and Curie-Weiss temperature $\Theta_{CW}$ = -0.55(4) K. The heat capacity measurements show a broad anomaly at low temperatures that is attributed to the presence of a low-energy Einstein mode with characteristic temperature $\Theta_E$ = 44 K, approximately twice as high as in the isostructural 'Einstein solid' VAl$_{10.1}$.",1609.07161v1 2020-05-11,Crystal Structure and Thermoelectric Transport Properties of As-Doped Layered Pnictogen Oxyselenides NdO0.8F0.2Sb1-xAsxSe2,"We report the synthesis and thermoelectric transport properties of As-doped layered pnictogen oxyselenides NdO0.8F0.2Sb1-xAsxSe2 (x < 0.7), which are predicted to show high-performance thermoelectric properties based on first-principles calculation. The crystal structure of these compounds belongs to the tetragonal P4/nmm space group (No. 129) at room temperature. The lattice parameter c decreases with increasing x, while a remains almost unchanged among the samples. Despite isovalent substitution of As for Sb, electrical resistivity significantly rises with increasing x. Very low thermal conductivity of less than 0.8 W/mK is observed at temperatures between 300 and 673 K for all the examined samples. For As-doped samples, the thermal conductivity further decreases above 600 K. Temperature-dependent synchrotron X-ray diffraction indicates that an anomaly also occurs in the c-axis length at around 600 K, which may relate to the thermal transport properties.",2005.04836v1 2020-05-17,Paramagnetic resonance in La2NiMnO6 probed by impedance and lock-in detection techniques,"We report the detection of paramagnetic resonance in the double perovskite La2NiMnO6 at room temperature for microwave magnetic fields with frequencies, f = 1 GHz to 5 GHz, using two cavity-less methods. We use an indirect impedance method which makes use of a radio frequency impedance analyzer and a folded copper strip coil for the frequency range f = 1 to 2.2 GHz. In this method, when an applied dc magnetic field is swept, high-frequency resistance of the strip coil exhibits a sharp peak and the reactance curve crosses zero exhibiting resonance. A lock-in based broadband setup using a coplanar waveguide for microwave excitation was used for f = 2 to 5 GHz The resonance fields (Hr) obtained from both the techniques increase linearly with frequency and a large spectroscopic g-factor, equal to 2.1284, which supports the presence of Ni2+ cation with strong spin-orbit coupling. Line shape analysis and analytical fitting were performed to characterize the material in terms of its initial susceptibility and damping parameters.",2005.08142v1 2020-05-19,Molecular beam epitaxy growth of nonmagnetic Weyl semimetal LaAlGe thin film,"Here, we report a detailed method of growing LaAlGe, a non-magnetic Weyl semimetal, thin film on silicon(100) substrates by molecular beam epitaxy and their structural and electrical characterizations. 50 nm thick LaAlGe films were deposited and annealed for 16 hours in situ at a temperature 793 K. As-grown high-quality films showed uniform surface topography and near ideal stoichiometry with a body-centered tetragonal crystal structure. Temperature-dependent longitudinal resistivity can be understood with dominant interband s-d electron-phonon scattering in the temperature range 5-40 K. Hall measurements confirmed the semimetallic nature of the films with electron dominated charge carrier density near 7.15*10^21 cm^-3 at 5 K.",2005.09695v1 2020-07-13,One nanometer HfO$_2$-based ferroelectric tunnel junctions on silicon,"In ferroelectric materials, spontaneous symmetry breaking leads to a switchable electric polarization, which offers significant promise for nonvolatile memories. In particular, ferroelectric tunnel junctions (FTJs) have emerged as a new resistive switching memory which exploit polarization-dependent tunnel current across a thin ferroelectric barrier. Here we demonstrate FTJs with CMOS-compatible Zr-doped HfO$_2$ (Zr:HfO$_2$) ferroelectric barriers of just 1 nm thickness, grown by atomic layer deposition on silicon. These 1 nm Zr:HfO$_2$ tunnel junctions exhibit large polarization-driven electroresistance (19000$\%$), the largest value reported for HfO$_2$-based FTJs. In addition, due to just a 1 nm ferroelectric barrier, these junctions provide large tunnel current (> 1 A/cm$^2$) at low read voltage, orders of magnitude larger than reported thicker HfO$_2$-based FTJs. Therefore, our proof-of-principle demonstration provides an approach to simultaneously overcome three major drawbacks of prototypical FTJs: a Si-compatible ultrathin ferroelectric, large electroresistance, and large read current for high-speed operation.",2007.06182v1 2020-08-03,Energy gap tuning and gate-controlled topological phase transition in InAs/In$_{x}$Ga$_{1-x}$Sb composite quantum wells,"We report transport measurements of strained InAs/In$_{x}$Ga$_{1-x}$Sb composite quantum wells (CQWs) in the quantum spin Hall phase, focusing on the control of the energy gap through structural parameters and an external electric field. For highly strained CQWs with $x = 0.4$, we obtain a gap of 35 meV, an order of magnitude larger than that reported for binary InAs/GaSb CQWs. Using a dual-gate configuration, we demonstrate an electrical-field-driven topological phase transition, which manifests itself as a re-entrant behavior of the energy gap. The sizeable energy gap and high bulk resistivity obtained in both the topological and normal phases of a single device open the possibility of electrical switching of the edge transport.",2008.00664v1 2020-08-15,Microwave AC voltage induced phase change in Sb$_2$Te$_3$ nanowires,"Scaling information bits to ever smaller dimensions is a dominant drive for information technology (IT). Nanostructured phase change material emerges as a key player in the current green-IT endeavor with low power consumption, functional modularity and promising scalability. In this work, we present the demonstration of microwave AC voltage induced phase change phenomenon at 3 GHz in single Sb$_2$Te$_3$ nanowires. The resistance change by a total of 6 - 7 orders of magnitude is evidenced by a transition from the crystalline metallic to the amorphous semiconducting phase, which is cross-examined by temperature dependent transport measurement and high-resolution electron microscopy analysis. This discovery could potentially tailor multi-state information bit encoding and discrimination along a single nanowire, rendering technology advancement for neuro-inspired computing devices.",2008.06666v1 2020-10-23,Observation of photoelectric nonvolatile memory and oscillations in VO2 at room temperature,"Vanadium dioxide (VO2) is a phase change material that can reversibly change between high and low resistivity states through electronic and structural phase transitions. Thus far, VO2 memory devices have essentially been volatile at room temperature, and nonvolatile memory has required non-ambient surroundings (e.g., elevated temperatures, electrolytes) and long write times. Here, we report the first observation of optically addressable nonvolatile memory in VO2 at room temperature with a readout by voltage oscillations. The read and write times had to be kept shorter than about 150 {\mu}s. The writing of the memory and onset of the voltage oscillations had a minimum optical power threshold. This discovery demonstrates the potential of VO2 for new computing devices and architectures, such as artificial neurons and oscillatory neural networks.",2010.12531v1 2020-11-17,Effect of Surface Treatment on High-Temperature Oxidation Behavior of IN 713C,"The effects of surface preparations on oxidation kinetics and oxide scale morphology for the commercially available Ni-based superalloy IN 713C have been investigated. The ground and polished samples were exposed in air at 800-1100C. The ground specimens were found to demonstrate lower oxidation kinetics compared to those after polishing. The grinding also affected the oxide scale morphology, resulting in a protective alumina scale, while the polished samples developed Ni-/Cr-rich mixed oxides on the surface. Better oxidation resistance of the ground surfaces is related to a higher concentration of defects in the nearsurface region introduced by cold working. These defects facilitate the outward transport of the scaleforming element Al and thus are beneficial for protective oxidation. The oxidation mechanism at lower temperatures was introduced. The model based on the generalized Darken method and multiphase approximation was proposed.",2011.08910v1 2021-02-01,Resistive transition of hydrogen-rich superconductors,"Critical temperature, $T_c$, and the transition width, $\Delta$$T_c$, are two primary parameters of the superconducting transition. The latter parameter reflects the superconducting state disturbance originating from the thermodynamic fluctuations, atomic disorder, applied magnetic field, the presence of secondary crystalline phases, applied pressure, etc. Recently, Hirsch and Marsiglio (2020 arXiv:2012.12796) performed an analysis of the transition width in several near-room-temperature superconductors (NRTS) and reported that the reduced transition width, $\Delta$$T_c$$/$$T_c$, in these materials does not follow a conventional trend of transition width broadening on applied magnetic field observed in low- and high-$T_c$ superconductors. Here we present thorough mathematical analysis of the magnetoresistive data, $\it{R(T,B)}$, for the high-entropy alloy $(ScZrNb)_{0.65}$$[RhPd]_{0.35}$ and hydrogen-rich superconductors of Im-3m-$H_{3}S$, C2/m-$LaH_{10}$ and P63/mmc-$CeH_9$. We found that the reduced transition width, $\Delta$$T_c$$/$$T_c$, in these materials does follow a conventional broadening trend on applied magnetic field.",2102.00946v3 2021-02-10,Evidence of damage in carbon fibre composite tiles joined to a metallic heat sink under high heat flux fatigue,"The two years experience with Active Metal Casting flat bonds shows that this technology is suitable for the heat fluxes expected in Tore Supra (10 MW/m${}^2$). Tests were pursued up to 3330 cycles, with elements still functional. At higher heat fluxes, fatigue damage is observed, but the bond resists remarkably well with no tile detachment. Examination of such deliberately damaged bonds showed distributed cracking, proving the absence of any weak link. The limitations to those higher heat fluxes are more related to the design and the base materials than to the bond itself.",2102.05316v1 2021-03-14,Electron-beam Floating-zone Refined UCoGe,"The interplay between unconventional superconductivity and quantum critical ferromagnetism in the U-Ge compounds represents an open problem in strongly correlated electron systems. Sample quality can have a strong influence on both of these ordered states in the compound UCoGe, as is true for most unconventional superconductors. We report results of a new approach at UCoGe crystal growth using a floating-zone method with potential for improvements of sample quality and size as compared with traditional means such as Czochralski growth. Single crystals of the ferromagnetic superconductor UCoGe were produced using an ultra-high vacuum electron-beam floating-zone refining technique. Annealed single crystals show well-defined signatures of bulk ferromagnetism and superconductivity at $T_c \sim$2.6 K and $T_s \sim$0.55 K, respectively, in the resistivity and heat capacity. Scanning electron microscopy of samples with different surface treatments shows evidence of an off-stoichiometric uranium rich phase of UCoGe collected in cracks and voids that might be limiting sample quality.",2103.08000v1 2021-03-24,Large Nernst effect and field enhanced transversal ZT in ZrTe5,"Thermoelectric materials can recover electrical energy from waste heat and vice versa, which are of great significance in green energy harvesting and solid state refrigerator. The thermoelectric figure of merit (zT) quantifies the energy conversion efficiency, and a large Seebeck or Nernst effect is crucial for the development of thermoelectric devices. Here we present a significantly large Nernst thermopower in topological semimetal ZrTe5, which is attributed to both strong Berry curvature and bipolar transport. The largest in-plane S_xy (when B//b) approaches 1900 {\mu}V/K at T=100K and B=13T, and the out-of-plane S_xz (when B//c) reaches 5000 {\mu}V/K. As a critical part of z_N T, the linearly increased in-plane S_xy and resistivity \r{ho}_yy regard to B induces an almost linear increasing transversal z_N T without saturate under high fields. The maximum z_N T of 0.12 was obtained at B=13 T and T= 120K, which significantly surmounts its longitudinal counterpart under the same condition.",2103.13069v1 2021-03-26,Large Microwave Inductance of Granular Boron-Doped Diamond Superconducting Films,"Boron-doped diamond granular thin films are known to exhibit superconductivity with an optimal critical temperature of Tc = 7.2K. Here we report the measured complex surface impedance of Boron-doped diamond films in the microwave frequency range using a resonant technique. Experimentally measured inductance values are in good agreement with estimates obtained from the normal state sheet resistance of the material. The magnetic penetration depth temperature dependence is consistent with that of a fully-gapped s-wave superconductor. Boron-doped diamond films should find application where high kinetic inductance is needed, such as microwave kinetic inductance detectors and quantum impedance devices.",2103.14738v3 2021-06-25,An estimate for thermal diffusivity in highly irradiated tungsten using Molecular Dynamics simulation,"The changing thermal conductivity of an irradiated material is among the principal design considerations for any nuclear reactor, but at present few models are capable of predicting these changes starting from an arbitrary atomistic model. Here we present a simple model for computing the thermal diffusivity of tungsten, based on the conductivity of the perfect crystal and resistivity per Frenkel pair, and dividing a simulation into perfect and athermal regions statistically. This is applied to highly irradiated microstructures simulated with Molecular Dynamics. A comparison to experiment shows that simulations closely track observed thermal diffusivity over a range of doses from the dilute limit of a few Frenkel pairs to the high dose saturation limit at 3 displacements per atom (dpa).",2106.13666v2 2021-07-15,Microstructure manipulation by laser-surface remelting of a full-Heusler compound to enhance thermoelectric properties,"There is an increasing reckoning that the thermoelectric performance of a material is dependent on its microstructure. However, the microstructure-properties relationship often remains elusive, in part due to the complexity of the hierarchy and scales of features that influence transport properties. Here, we focus on the promising Heusler-Fe2VAl compound. We directly correlate microstructure and local properties, using advanced scanning electron microscopy methods including in-situ four-point-probe technique for electron transport measurements. The local thermal conductivity is investigated by scanning thermal microscopy. Finally, atom probe tomography provides near-atomic scale compositional analysis. To locally manipulate the microstructure, we use laser surface remelting. The rapid quenching creates a complex microstructure with a high density of dislocations and small, elongated grains. We hence showcase that laser surface remelting can be employed to manipulate the microstructure to reduce the thermal conductivity and electrical resistivity, leading to a demonstrated enhancement of the thermoelectric performance at room temperature.",2107.07327v1 2021-07-29,Breakdown of the topological protection by cavity vacuum fields in the integer quantum Hall effect,"The control of the electronic properties of materials via the vacuum fields of cavity electromagnetic resonators is one of the emerging frontiers of condensed matter physics. We show here that the enhancement of vacuum field fluctuations in subwavelength split-ring resonators dramatically affects arguably one of the most paradigmatic quantum protectorates, namely the quantum Hall electron transport in high-mobility 2D electron gases. The observed breakdown of the topological protection of the integer quantum Hall effect is interpreted in terms of a long-range cavity-mediated electron hopping where the anti-resonant terms of the light-matter coupling finally result into a finite resistivity induced by the vacuum fluctuations. The present experimental platform can be used for any 2D material and provides new ways to manipulate electron phases in matter thanks to vacuum-field engineering",2107.14145v1 2021-09-03,Quantum anomalous Hall edge channels survive up to the Curie temperature,"Achieving metrological precision of quantum anomalous Hall resistance quantization at zero magnetic field so far remains limited to temperatures of the order of 20 mK, while the Curie temperature in the involved material is as high as 20 K. The reason for this discrepancy remains one of the biggest open questions surrounding the effect, and is the focus of this article. Here we show, through a careful analysis of the non-local voltages on a multi-terminal Corbino geometry, that the chiral edge channels continue to exist without applied magnetic field up to the Curie temperature of bulk ferromagnetism of the magnetic topological insulator, and that thermally activated bulk conductance is responsible for this quantization breakdown. Our results offer important insights on the nature of the topological protection of these edge channels, provide an encouraging sign for potential applications, and establish the multi-terminal Corbino geometry as a powerful tool for the study of edge channel transport in topological materials.",2109.01463v1 2021-11-03,Insulator-to-superconductor transition in quasi-one-dimensional HfS3 under pressure,"Various transition metal trichalcogenides (TMTC) show the charge-density-wave and superconductivity, which provide an ideal platform to study the correlation between these two orderings and the mechanism of superconductivity. Currently, almost all metallic TMTC compounds can show superconductivity either at ambient pressure or at high pressure. However, most TMTC compounds are semiconductors and even insulators. Does the superconductivity exist in any non-metal TMTC compound? In this work, we managed to manipulate the electronic behavior of highly insulating HfS3 in term of pressure. HfS3 underwent an insulator-semiconductor transition near 17 GPa with a band gap reduce of ~1 eV. The optical absorption and Raman measurement provide the consistent results, suggesting the structural origin of the electronic transition. Upon further compression, HfS3 becomes a superconductor. The superconducting transition was initialized as early as 50.6 GPa and the zero-resistance is reached above 91.2 GPa. The superconducting behavior is further confirmed by both the magnetic field effect and current effect. This work sheds the light that all TMTC may be superconductors, and opens a new avenue to explore the abundant emergence phenomena in TMTC material family.",2111.02060v1 2021-11-16,Ultrathin ferrimagnetic GdFeCo films with very low damping,"Ferromagnetic materials dominate as the magnetically active element in spintronic devices, but come with drawbacks such as large stray fields, and low operational frequencies. Compensated ferrimagnets provide an alternative as they combine the ultrafast magnetization dynamics of antiferromagnets with a ferromagnet-like spin-orbit-torque (SOT) behavior. However to use ferrimagnets in spintronic devices their advantageous properties must be retained also in ultrathin films (t < 10 nm). In this study, ferrimagnetic Gdx(Fe87.5Co12.5)1-x thin films in the thickness range t = 2-20 nm were grown on high resistance Si(100) substrates and studied using broadband ferromagnetic resonance measurements at room temperature. By tuning their stoichiometry, a nearly compensated behavior is observed in 2 nm Gdx(Fe87.5Co12.5)1-x ultrathin films for the first time, with an effective magnetization of Meff = 0.02 T and a low effective Gilbert damping constant of {\alpha} = 0.0078, comparable to the lowest values reported so far in 30 nm films. These results show great promise for the development of ultrafast and energy efficient ferrimagnetic spintronic devices.",2111.08768v1 2021-12-06,Sliding Ferroelectric Tunnel Junctions,"Very recently, ferroelectric polarization in staggered bilayer hexagonal boron nitride (BBN) and its novel sliding inversion mechanism was reported experimentally (Science 2021, 372, 1458; 2021, 372, 1462), which paves a new way to realize van der Waals (vdW) ferroelectric devices with new functionalities. Here, we develop vdW sliding ferroelectric tunnel junctions (FTJs) using the sliding ferroelectric BBN unit as ultrathin barriers and explore their transport properties with different ferroelectric states and metal contacts via the first principles. It is found that the electrode/BBN contact electric field quenches the ferroelectricity in the staggered BBN, resulting a very small tunnelling electroresistance (TER). Inserting high-mobility 2D materials between Au and BN can restore the BBN ferroelectricity, reaching a giant TER of ~10,000% in sliding FTJs. We finally investigate the metal-contact and thickness effect on the tunnelling property of sliding FTJs. The giant TER and multiple non-volatile resistance states in vdW sliding FTJs show the promising applications in voltage-controlled nano-memories with ultrahigh storage density.",2112.02886v1 2022-06-06,Enhancement of superconductivity on the verge of a structural instability in isovalently doped $β$-ThRh$_{1-x}$Ir$_{x}$Ge,"$\beta$-ThRhGe, the high-temperature polymorph of ThRhGe, is isostructural to the well-known ferromagnetic superconductor URhGe. However, contrary to URhGe, $\beta$-ThRhGe is nonmagnetic and undergoes an incomplete structural phase transition at 244 K, followed by a superconducting transition below 3.36 K. Here we show that the isovalent substitution of Ir for Rh leads to a strong enhancement of superconductivity by suppressing the structural transition. At $x$ = 0.5, where the structural transition disappears, $T_{\rm c}$ reaches a maximum of 6.88 K. The enhancement of superconductivity is linked to the proximity to a structural quantum critical point at this Ir concentration, as suggested by the analysis of thermodynamic as well as resistivity data. First principles calculations indicate that the Ir doping has little effect on the electronic band dispersion near the Fermi level. $\beta$-ThRh$_{1-x}$Ir$_{x}$Ge thus provides an excellent platform to study the interplay between superconductivity and structural quantum criticality in actinide-containing compounds.",2206.02364v1 2022-06-21,HR-EBSD analysis of in situ stable crack growth at the micron scale,"Understanding the local fracture resistance of microstructural features. such as brittle inclusions, coatings, and interfaces at the microscale under complex loading conditions is critical for microstructure-informed design of materials. In this study, a novel approach has been formulated to decompose the J-integral evaluation of the elastic energy release rate to the three-dimensional stress intensity factors directly from experimental measurements of the elastic deformation gradient tensors of the crack field by in situ high (angular) resolution electron backscatter diffraction (HR-EBSD). An exemplar study is presented of a quasi-static crack, inclined to the observed surface, propagating on low index {hkl} planes in a (001) single crystal silicon wafer.",2206.10243v2 2022-10-01,Surface modulation of metal-organic frameworks for on-demand photochromism in the solid state,"Organic photoswitchable molecules have struggled in solid state form to fulfill their remarkable potential, in terms of photoswitching performance and long-term stability when compared to their inorganic counterparts. We report the concept of non-electron deficient host's surface with optimal porosity and hydrophobicity, as a priori strategy to design photoefficient organic solid-state photochromic materials with outstanding mechanical robustness. When exposed to a light stimulus including natural sunlight, the photoswitchable nanocomposite changes color promptly and reversibly, in a matter of seconds along with excellent photo-fatigue resistance, which are on a par with inorganic photochromes. Exemplars of commercially viable prototypes that are optically clear, comprising smart windows, complex photochromic sculptures, and self-erasing rewritable devices, were engineered by direct blending with resilient polymers; particularly, the use of high-stiffness polymer (> 2 GPa) is no longer an insurmountable challenge. Finally, photochromic films with anticounterfeiting features could be manufactured through precision inkjet printing of nanocrystals.",2210.00241v1 2022-10-06,Fracture behavior of MOF monoliths revealed by nanoindentation and nanoscratch,"Monolithic metal-organic frameworks (MOFs) represent a promising solution for the industrial implementation of this emerging class of multifunctional materials, due to their structural stability. When compared to MOF powders, monoliths exhibit other intriguing properties like hierarchical porosity, that significantly improves volumetric adsorption capacity. The mechanical characterization of MOF monoliths plays a pivotal role in their industrial expansion, but so far, several key aspects remain unclear. In particular, the fracture behavior of MOF monoliths has not been explored. In this work, we studied the initiation and propagation of cracks in four prototypical MOF monoliths, namely ZIF-8, HKUST-1, MIL-68 and MOF-808. We observed that shear faults inside the contact area represent the main failure mechanism of MOF monoliths and are the source of radial cracks. MIL-68 and MOF-808 showed a remarkably high resistance to cracking, which can be ascribed to their consolidated nanostructure.",2210.03219v1 2022-10-26,Thermoelectric properties in semimetals with inelastic electron-hole scattering,"We present systematic theoretical results on thermoelectric effects in semimetals based on the variational method of the linearized Boltzmann equation. Inelastic electron-hole scattering is known to play an important role in the unusual transport of semimetals, including the broad $T^2$ temperature dependence of the electrical resistivity and the strong violation of the Wiedemann-Franz law. By treating the inelastic electron-hole scattering more precisely beyond the relaxation time approximation, we show that the Seebeck coefficient when compensated depends on the screening length of the Coulomb interaction as well as the Lorenz ratio (the ratio of thermal to electric conductivity due to electrons divided by temperature). It is found that deviations from the compensation condition significantly increase the Seebeck coefficient, along with crucial suppressions of the Lorenz ratio. The result indicates that uncompensated semimetals with the electron-hole scattering have high thermoelectric efficiency when the phonon contribution to thermal conductivity is suppressed.",2210.14825v2 2023-01-10,Depolarization Induced III-V Triatomic Layers with Tristable Polarization States,"The integration of ferroelectrics that exhibit high dielectric, piezoelectric, and thermal susceptibilities with the mainstream semiconductor industry will enable novel device types for widespread applications, and yet there are few silicon-compatible ferroelectrics suitable for device downscaling. We demonstrate with first-principles calculations that the enhanced depolarization field at the nanoscale can be utilized to soften unswitchable wurtzite III-V semiconductors, resulting in ultrathin two-dimensional (2D) sheets possessing reversible polarization states. A 2D sheet of AlSb consisting of three atomic planes is identified to host both ferroelectricity and antiferroelectricity, and the tristate switching is accompanied by a metal-semiconductor transition. The thermodynamics stability and potential synthesizability of the triatomic layer are corroborated with phonon spectrum calculations, ab initio molecular dynamics, and variable-composition evolutionary structure search. We propose a 2D AlSb-based homojunction field effect transistor that supports three distinct and nonvolatile resistance states. This new class of III-V semiconductor-derived 2D materials with dual ferroelectricity and antiferroelectricity opens up the possibility for nonvolatile multibit-based integrated nanoelectronics.",2301.03876v1 2023-01-11,Direct imaging of local atomic structures in zeolite using novel low-dose scanning transmission electron microscopy,"Zeolites have been used in industrial applications such as catalysts, ion exchangers, and molecular sieves because of their unique porous atomic structures. However, the direct observation of zeolitic local atomic structures via electron microscopy is difficult owing to their low resistance to electron irradiation. Subsequently, the fundamental relationships between these structures and their properties remain unclear. A novel low-electron-dose imaging technique, optimum bright-field scanning transmission electron microscopy (OBF STEM) has recently been developed. It reconstructs images with a high signal-to-noise ratio and a dose efficiency approximately two orders of magnitude higher than that of conventional methods. Herein, we performed low-dose atomic-resolution OBF STEM observations of an FAU-type zeolite, effectively visualizing all the atomic sites in its framework. Additionally, the complex local atomic structure of the twin boundaries in the zeolite was directly characterized. The results of this study facilitate the characterization of the local atomic structures in many electron-beam-sensitive materials.",2301.04377v1 2023-04-25,Simulations of Magnetization Reversal in FM/AFM Bilayers With THz Frequency Pulses,"It is widely known that antiferromagnets (AFMs) display a high frequency response in the terahertz (THz) range, which opens up the possibility for ultrafast control of their magnetization for next generation data storage and processing applications. However, because the magnetization of the different sublattices cancel, their state is notoriously difficult to read. One way to overcome this is to couple AFMs to ferromagnets - whose state is trivially read via magneto-resistance sensors. Here we present conditions, using theoretical modelling, that it is possible to switch the magnetization of an AFM/FM bilayer using THz frequency pulses with moderate field amplitude and short durations, achievable in experiments. Consistent switching is observed in the phase diagrams for an order of magnitude increase in the interface coupling and a tripling in the thickness of the FM layer. We demonstrate a range of reversal paths that arise due to the combination of precession in the materials and the THz-induced fields. Our analysis demonstrates that the AFM drives the switching and results in a much higher frequency dynamics in the FM due to the exchange coupling at the interface. The switching is shown to be robust over a broad range of temperatures relevant for device applications.",2304.12969v1 2023-05-24,A new class of carbon stabilized austenitic steels resistant to hydrogen embrittlement,"High strength steels are susceptible to H-induced failure, which is typically caused by the presence of diffusible H in the microstructure. The diffusivity of H in austenitic steels with fcc crystal structure is slow. The austenitic steels are hence preferred for applications in the hydrogen-containing atmospheres. However, the fcc structure of austenitic steels is often stabilized by the addition of Ni, Mn or N, which are relatively expensive alloying elements to use. Austenite can kinetically also be stabilized by using C. Here, we present an approach applied to a commercial cold work tool steel, where we use C to fully stabilize the fcc phase. This results in a microstructure consisting of only austenite and an M7C3 carbide. An exposure to H by cathodic hydrogen charging exhibited no significant influence on the strength and ductility of the C stabilized austenitic steel. While this material is only a prototype based on an existing alloy of different purpose, it shows the potential for low-cost H-resistant steels based on C stabilized austenite.",2305.15290v3 2023-06-17,Pseudogap behavior in charge density wave kagome material ScV$_6$Sn$_6$ revealed by magnetotransport measurements,"Over the last few years, significant attention has been devoted to studying the kagome materials AV$_3$Sb$_5$ (A = K, Rb, Cs) due to their unconventional superconductivity and charge density wave (CDW) ordering. Recently ScV$_6$Sn$_6$ was found to host a CDW below $\approx$90K, and, like AV$_3$Sb$_5$, it contains a kagome lattice comprised only of V ions. Here we present a comprehensive magnetotransport study on ScV$_6$Sn$_6$. We discovered several anomalous transport phenomena above the CDW ordering temperature, including insulating behavior in interlayer resistivity, a strongly temperature-dependent Hall coefficient, and violation of Kohler's rule. All these anomalies can be consistently explained by a progressive decrease in carrier densities with decreasing temperature, suggesting the formation of a pseudogap. Our findings suggest that high-temperature CDW fluctuations play a significant role in determining the normal state electronic properties of ScV$_6$Sn$_6$.",2306.10230v1 2023-07-12,Monolithic Selenium/Silicon Tandem Solar Cells,"Selenium is experiencing renewed interest as a promising candidate for the wide bandgap photoabsorber in tandem solar cells. However, despite the potential of selenium-based tandems to surpass the theoretical efficiency limit of single junction devices, such a device has never been demonstrated. In this study, we present the first monolithically integrated selenium/silicon tandem solar cell. Guided by device simulations, we investigate various carrier-selective contact materials and achieve encouraging results, including an open-circuit voltage of V$_\text{oc}$=1.68 V from suns-V$_\text{oc}$ measurements. The high open-circuit voltage positions selenium/silicon tandem solar cells as serious contenders to the industrially dominant single junction technologies. Furthermore, we quantify a pseudo fill factor of more than 80% using injection-level-dependent open-circuit voltage measurements, indicating that a significant fraction of the photovoltaic losses can be attributed to parasitic series resistance. This work provides valuable insights into the key challenges that need to be addressed for realizing higher efficiency selenium/silicon tandem solar cells.",2307.05996v1 2023-10-09,Colossal c-axis response and lack of rotational symmetry breaking within the kagome plane of the CsV$_3$Sb$_5$ superconductor,"The kagome materials AV4$_3$Sb$_5$ (A = K, Rb, Cs) host an intriguing interplay between unconventional superconductivity and charge-density-waves. Here, we investigate CsV$_3$Sb$_5$ by combining high-resolution thermal-expansion, heat-capacity and electrical resistance under strain measurements. We directly unveil that the superconducting and charge-ordered states strongly compete, and that this competition is dramatically influenced by tuning the crystallographic c-axis. In addition, we report the absence of additional bulk phase transitions within the charge-ordered state, notably associated with rotational symmetry-breaking within the kagome planes. This suggests that any breaking of the C$_6$ invariance occurs via different stacking of C$_6$-symmetric kagome patterns. Finally, we find that the charge-density-wave phase exhibits an enhanced A$_{1g}$-symmetric elastoresistance coefficient, whose large increase at low temperature is driven by electronic degrees of freedom.",2310.06102v1 2023-10-15,Parabolic Vector Focus Wave Modes,"Weber-type parabolic beams have a transverse intensity profile, which is parabolically-shaped and can be flexibly controlled. On the other hand, this type of beams belongs to the family of the so-called nondiffracting beams and have properties, promising for applications where the shape of the beam is of an importance. Vector electromagnetic theory has to be introduced in order to fully describe optical beams inside a high numerical aperture system, where the angles of the spatial spectra are large. We introduce here parabolic vector focus wave modes (FWM), which are both resistant to diffraction and to material dispersion. We employ here a spectral approach and investigate durations of parabolic vector FWMs in the femtosecond region. Two cases of transverse electric and transverse magnetic modes are introduced and both standing and traveling types of waves are considered. We demonstrate how the angular dispersion affects the pulse shape and its properties. Parabolic vector FWMs are studied in a transparent dielectric media (sapphire), which is widely used as laser processed material.",2310.09896v1 2023-11-09,Single-Atom Control of Arsenic Incorporation in Silicon for High-Yield Artificial Lattice Fabrication,"Artificial lattices constructed from individual dopant atoms within a semiconductor crystal hold promise to provide novel materials with tailored electronic, magnetic, and optical properties. These custom engineered lattices are anticipated to enable new, fundamental discoveries in condensed matter physics and lead to the creation of new semiconductor technologies including analog quantum simulators and universal solid-state quantum computers. In this work, we report precise and repeatable, substitutional incorporation of single arsenic atoms into a silicon lattice. We employ a combination of scanning tunnelling microscopy hydrogen resist lithography and a detailed statistical exploration of the chemistry of arsine on the hydrogen terminated silicon (001) surface, to show that single arsenic dopants can be deterministically placed within four silicon lattice sites and incorporated with 97$\pm$2% yield. These findings bring us closer to the ultimate frontier in semiconductor technology: the deterministic assembly of atomically precise dopant and qubit arrays at arbitrarily large scales.",2311.05752v1 2023-11-26,"Quantum oscillations in kagome metals (Ti, Zr, Hf)V6Sn6 at Van Hove filling","Kagome materials have recently drawn great attention due to the interplay between nontrivial band topology, electron correlations, and Van Hove singularities related many-body orders. Here we report three new vanadium-based kagome metals, TiV6Sn6, ZrV6Sn6, and HfV6Sn6, and conduct a comprehensive investigation of their structural, magnetic, and electrical transport properties. All three compounds exhibit large unsaturated magnetoresistances and multiband Hall effects at low temperatures, indicating the existence of multiple highly mobile carriers. Both the diagonal and off-diagonal resistivity show quantum oscillations with nontrivial Berry phases and high quantum mobilities. First-principles calculations together with quantum oscillation analyses suggest the Van Hove singularities at the M point for the three compounds all located in close vicinity of the Fermi level, and there also exist multiple topological nontrivial band crossings, including a nodal ring and a massive Dirac cone. Our work extends the kagome AM6X6 family and paves the way for searching possible Van Hove physics in the V kagome lattice.",2311.15239v2 2023-12-14,Long-Range Structural Order in a Hidden Phase of Ruddlesden-Popper Bilayer Nickelate La$_3$Ni$_2$O$_7$,"The recent discovery of superconductivity in Ruddlesden-Popper bilayer nickelate, specifically La$_3$Ni$_2$O$_7$, has generated significant interest in the exploration of high-temperature superconductivity within this material family. In this study, we present the crystallographic and electrical resistivity properties of two distinct Ruddlesden-Popper nickelates: the bilayer La$_3$Ni$_2$O$_7$ (referred to as 2222-phase) and a previously uncharacterized phase, La$_3$Ni$_2$O$_7$ (1313-phase). The 2222-phase is characterized by a pseudo $F$-centered orthorhombic lattice, featuring bilayer perovskite [LaNiO$_3$] layers interspaced by rock salt [LaO] layers, forming a repeated ...2222... sequence. Intriguingly, the 1313-phase, which displays semiconducting properties, crystallizes in the $Cmmm$ space group and exhibits a pronounced predilection for a $C$-centered orthorhombic lattice. Within this structure, the perovskite [LaNiO$_3$] layers exhibit a distinctive long-range ordered arrangement, alternating between single- and trilayer configurations, resulting in a ...1313... sequence. This report contributes to novel insights into the crystallography and the structure-property relationship of Ruddlesden-Popper nickelates, paving the way for further investigations into their unique physical properties.",2312.09200v2 2024-03-11,Active Control of Bound States in the Continuum in Toroidal Metasurfaces,"The remarkable properties of toroidal metasurfaces, featuring ultrahigh-Q bound states in the continuum (BIC) resonances and nonradiating anapole modes, have garnered significant attention. The active manipulation of toroidal resonance characteristics offers substantial potential for advancing tunable metasurfaces. Our study specifically explores the application of vanadium dioxide, a widely used phase change material in active photonics and room-temperature bolometric detectors, to control BIC resonances in toroidal metasurfaces. The phase change transition of vanadium dioxide occurs in a narrow temperature range providing a large variation in material resistivity. Through heating thin film patches of vanadium dioxide integrated into a metasurface comprising gold split-ring resonators on a sapphire substrate, we achieve remarkable control over the amplitude and frequency of toroidal dipole BIC resonances due to their high sensitivity to losses present in the system. Breaking the symmetry of meta-atoms reveals enhanced tunability. The predicted maximum change in the amplitude of toroidal dipole BIC resonances reaches 14 dB with a temperature variation of approximately 10oC. The proposed tunable metasurface holds promise for various applications, including active photonic systems and room temperature bolometers.",2403.06345v1 2024-04-11,Hydrogen Trapping and Embrittlement in Metals -- A Review,"Hydrogen embrittlement in metals (HE) is a serious challenge for the use of high strength materials in engineering practice and a major barrier to the use of hydrogen for global decarbonization. Here we describe the factors and variables that determine HE susceptibility and provide an overview of the latest understanding of HE mechanisms. We discuss hydrogen uptake and how it can be managed. We summarize hydrogen trapping and the techniques used for its characterization. We also review literature that argues that hydrogen trapping can be used to decrease HE susceptibility. We discuss the future research that is required to advance the understanding of HE and hydrogen trapping and to develop HE-resistant alloys.",2404.07736v1 1999-07-23,Unconventional one-magnon scattering resistivity in half metals,"Low-temperature resistivity of half-metals is investigated. To date it has been discussed that the one-magnon scattering process in half-metals is irrelevant for low-temperature resistivity, due to the fully spin-polarized electronic structure at the ground state. If one takes into account the non-rigid-band behavior of the minority band due to spin fluctuations at finite temperatures, however, the unconventional one-magnon scattering process is shown to be most relevant and gives T^3 dependence in resistivity. This behavior may be used as a crucial test in the search for half-metallic materials which are potentially important for applications. Comparison with resistivity data of La_1-x Sr_x MnO_3 as candidates for half-metals shows good agreement.",9907363v2 2002-05-27,Superconductivity of epsilon-Fe: complete resistive transition,"Last year, iron was reported to become superconducting at temperatures below 2K and pressures between 15 and 30 GPa. The evidence presented was a weak resistivity drop, suppressed by a magnetic field above 0.2 T, and a small Meissner signal. However, a compelling demonstration, such as the occurrence of zero resistance, was lacking. Here we report the measurement of a complete resistive transition at 22.2 GPa with an onset slightly above 2 K in two very pure samples of iron, of different origins. The superconductivity appears unusually sensitive to disorder, developing only when the electronic mean free path is above a threshold value, while the normal state resistivity is characteristic of a nearly ferromagnetic metal.",0205557v1 2002-06-08,Diffusion theory of spin injection through resistive contacts,"Insertion of a resistive contact between a ferromagnetic metal and a semiconductor microstructure is of critical importance for achieving efficient spin injection into a semiconductor. However, the equations of the diffusion theory are rather cumbersome for the junctions including such contacts. A technique based on deriving a system of self-consistent equations for the coefficients of spin injection, ""gamma"", through different contacts are developed. These equations are concise when written in the proper notations. Moreover, the resistance of a two-contact junction can be expressed in terms of ""gamma""'s of both contacts. This equation makes calculating the spin valve effect straightforward, allows to find an explicit expression for the junction resistance and to prove that its nonequilibrium part is positive. Relation of these parameters to different phenomena like spin-e.m.f. and the junction transients is established. Comparative effect of the Coulomb screening on different parameters is clarified. It is also shown that the spin non-conservation in a contact can have a dramatic effect on the non-equilibrium resistance of the junction.",0206129v2 2002-08-13,Resistance of multilayers with long length scale interfacial roughness,"The resistance of multilayers with interface roughness on a length scale which is large compared to the atomic spacing is computed in several cases via the Boltzmann equation. This type of roughness is common in magnetic multilayers. When the electronic mean free paths are small compared to the layer thicknesses, the current flow is non-uniform, and the resistance decreases in the Current-Perpendicular-to-Plane (CPP) configuration and increases in the Current-In-Plane (CIP) configuration. For mean free paths much longer than the layer thicknesses, the current flow is uniform, and the resistance increases in both the CPP and CIP configurations due to enhanced surface scattering. In both the CPP and CIP geometries, the giant magnetoresistance can be either enhanced or reduced by the presence of long length scale interface roughness depending on the parameters. Finally, the changes in the CPP and CIP resistivities due to increasing interface roughness are estimated using experimentally determined parameters.",0208251v1 2004-02-13,Superconducting Properties under Magnetic Field in Na$_{0.35}$CoO$_{2}{\cdot}1.3$H$_{2}$O Single Crystal,"We report the in-plane resistivity and magnetic susceptibility of the layered cobalt oxide Na$_{0.35}$CoO$_{2}{\cdot}1.3$H$_{2}$O single crystal. The temperature dependence of the resistivity shows metallic behavior from room temperature to the superconducting transition temperature $T_{c}$ of 4.5 K. Sharp resistive transition, zero resistivity and almost perfect superconducting volume fraction below $T_{c}$ indicate the good quality and the bulk superconductivity of the single crystal. The upper critical field $H_{c2}$ and the coherence length $\xi$ are obtained from the resistive transitions in magnetic field parallel to the c-axis and the $ab$-plane. The anisotropy of $\xi$, $\xi_{ab} / \xi_{c} =$ 12 nm/1.3 nm $\simeq$ 9.2, suggests that this material is considered to be an anisotropic three dimensional superconductor. In the field parallel to the $ab$-plane, $H_{c2}$ seems to be suppressed to the value of Pauli paramagnetic limit. It may indicate the spin singlet superconductivity in the cobalt oxide.",0402355v1 2004-03-22,"Electrical Transport Across an Individual Magnetic Domain Wall in (Ga,Mn)As Microdevices","Recent studies demonstrate that an individual magnetic domain wall (DW) can be trapped and reproducibly positioned within multiterminal (Ga,Mn)As microdevices. The electrical resistance obtained from such measurements is found to be measurably altered by the presence of this single entity. To elucidate these observations we develop a simple model for the electrical potential distribution along a multiterminal device in the presence of a single DW. This is employed to calculate the effect of a single DW upon the longitudinal and transverse resistance. The model provides very good agreement with experimental observations, and serves to highlight important deviations from simple theory. We show that measurements of transverse resistance along the channel permits establishing the position and the shape of the DW contained within it. An experimental scheme is developed that enables unambiguous extraction of the intrinsic DW resistivity. This permits the intrinsic contribution to be differentiated from resistivities originating from the bulk and from magnetic anisotropy - effects that are generally manifested as large backgrounds in the experiments.",0403547v1 2004-07-30,Occurrence of Hysteresis like behavior of resistance of $Sb_2 Te_3$ film in heating-cooling cycle,"Experimental observations of a peculiar behavior observed on heating and cooling ${\rm Sb_2Te_3}$ films at different heating and cooling rate are detailed. The film regained its original resistance, forming a closed loop, on the completion of the heating-cooling cycle which was reproducible for identical conditions of heating and cooling. The area enclosed by the loop was found to depend on (i) the thickness of the film, (ii) the heating rate, (iii) the maximum temperature to which film was heated and (iv) the cooling rate. The observations are explained on basis of model which considers the film to be a resultant of parallel resistances. The film's finite thermal conductivity gives rise to a temperature gradient along the thickness of the film, due to this and the temperature coefficient of resistance, the parallel combination of resistance changes with temperature. Difference in heating and cooling rates give different temperature gradient, which explains the observed hysteresis.",0407796v1 2004-08-03,Non-Gaussian Resistance Fluctuations in Disordered Materials,"We study the distribution of resistance fluctuations of conducting thin films with different levels of internal disorder. The film is modeled as a resistor network in a steady state determined by the competition between two biased processes, breaking and recovery of the elementary resistors. The fluctuations of the film resistance are calculated by Monte Carlo simulations which are performed under different bias conditions, from the linear regime up to the threshold for electrical breakdown. Depending on the value of the external current, on the level of disorder and on the size of the system, the distribution of the resistance fluctuations can exhibit significant deviations from Gaussianity. As a general trend, a size dependent, non universal distribution is found for systems with low and intermediate disorder. However, for strongly disordered systems, close to the critical point of the conductor-insulator transition, the non-Gaussianity persists when the size is increased and the distribution of resistance fluctuations is well described by the universal Bramwell-Holdsworth-Pinton distribution.",0408057v1 2007-02-26,Nonpolar resistance switching of metal/binary-transition-metal oxides/metal sandwiches: homogeneous/inhomogeneous transition of current distribution,"Exotic features of a metal/oxide/metal (MOM) sandwich, which will be the basis for a drastically innovative nonvolatile memory device, is brought to light from a physical point of view. Here the insulator is one of the ubiquitous and classic binary-transition-metal oxides (TMO), such as Fe2O3, NiO, and CoO. The sandwich exhibits a resistance that reversibly switches between two states: one is a highly resistive off-state and the other is a conductive on-state. Several distinct features were universally observed in these binary TMO sandwiches: namely, nonpolar switching, non-volatile threshold switching, and current--voltage duality. From the systematic sample-size dependence of the resistance in on- and off-states, we conclude that the resistance switching is due to the homogeneous/inhomogeneous transition of the current distribution at the interface.",0702564v1 2007-11-02,Effects of Ferromagnetic Magnetic Ordering and Phase Transition on the Resistivity of Spin Current,"It has been shown experimentally a long time ago that the magnetic ordering causes an anomalous behavior of the electron resistivity in ferromagnetic crystals. Phenomenological explanations based on the interaction between itinerant electron spins and lattice spins have been suggested to explain these observations. We show by extensive Monte Carlo simulation that this behavior is also observed for the resistivity of the spin current calculated as a function of temperature ($T$) from low-$T$ ordered phase to high-$T$ paramagnetic phase in a ferromagnet. We show in particular that across the critical region, the spin resistivity undergoes a huge peak. The origin of this peak is shown to stem from the formation of magnetic domains near the phase transition. The behavior of the resistivity obtained here is compared to experiments and theories. A good agreement is observed.",0711.0298v1 2008-01-29,Temperature Dependence of the Spin Resistivity in Ferromagnetic Thin Films,"The magnetic phase transition is experimentally known to give rise to an anomalous temperature-dependence of the electron resistivity in ferromagnetic crystals. Phenomenological theories based on the interaction between itinerant electron spins and lattice spins have been suggested to explain these observations. In this paper, we show by extensive Monte Carlo (MC) simulation the behavior of the resistivity of the spin current calculated as a function of temperature ($T$) from low-$T$ ordered phase to high-$T$ paramagnetic phase in a ferromagnetic film. We analyze in particular effects of film thickness, surface interactions and different kinds of impurities on the spin resistivity across the critical region. The origin of the resistivity peak near the phase transition is shown to stem from the existence of magnetic domains in the critical region. We also formulate in this paper a theory based on the Boltzmann's equation in the relaxation-time approximation. This equation can be solved using numerical data obtained by our simulations. We show that our theory is in a good agreement with our MC results. Comparison with experiments is discussed.",0801.4444v1 2008-02-19,"Advanced resistivity model for arbitrary magnetization orientation applied to a series of compressive- to tensile-strained (Ga,Mn)As layers","The longitudinal and transverse resistivities of differently strained (Ga,Mn)As layers are theoretically and experimentally studied as a function of the magnetization orientation. The strain in the series of (Ga,Mn)As layers is gradually varied from compressive to tensile using (In,Ga)As templates with different In concentrations. Analytical expressions for the resistivities are derived from a series expansion of the resistivity tensor with respect to the direction cosines of the magnetization. In order to quantitatively model the experimental data, terms up to the fourth order have to be included. The expressions derived are generally valid for any single-crystalline cubic and tetragonal ferromagnet and apply to arbitrary surface orientations and current directions. The model phenomenologically incorporates the longitudinal and transverse anisotropic magnetoresistance as well as the anomalous Hall effect. The resistivity parameters obtained from a comparison between experiment and theory are found to systematically vary with the strain in the layer.",0802.2635v1 2008-07-28,Current induced resistance change of magnetic tunnel junctions with ultra-thin MgO tunnel barriers,"Ultra-thin magnetic tunnel junctions with low resistive MgO tunnel barriers are prepared to examine their stability under large current stress. The devices show magnetoresistance ratios of up to 110 % and an area resistance product of down to 4.4 ohm micrometer squared. If a large current is applied, a reversible resistance change is observed, which can be attributed to two different processes during stressing and one relaxation process afterwards. Here, we analyze the time dependence of the resistance and use a simple model to explain the observed behavior. The explanation is further supported by numerical fits to the data in order to quantify the timescales of the involved phenomena.",0807.4422v1 2009-05-15,First-principles analysis of spin-disorder resistivity of Fe and Ni,"Spin-disorder resistivity of Fe and Ni and its temperature dependence are analyzed using noncollinear density functional calculations within the supercell method. Different models of thermal spin disorder are considered, including the mean-field approximation and the nearest-neighbor Heisenberg model. Spin-disorder resistivity is found to depend weakly on magnetic short-range order. If the local moments are kept frozen at their zero-temperature values, very good agreement with experiment is obtained for Fe, but for Ni the resistivity at elevated temperatures is significantly overestimated. Agreement with experiment for Fe is improved if the local moments are iterated to self-consistency. The overestimation of the resistivity for paramagnetic Ni is attributed to the reduction of the local moments down to 0.35 Bohr magnetons. Overall, the results suggest that low-energy spin fluctuations in Fe and Ni are better viewed as classical rotations of local moments rather than quantized spin fluctuations that would require an (S+1)/S correction.",0905.2606v1 2009-06-04,Resistivity of Graphene Nanoribbon Interconnects,"Graphene nanoribbon interconnects are fabricated, and the extracted resistivity is compared to that of Cu. It is found that the average resistivity at a given line-width (18nm$ $\rho_b$, where the $b$-axis parameter is shorter than the $a$-axis one) to that observed in the transition-metal doped iron arsenides ($\rho_a$ $<$ $\rho_b$). On the other hand, our results demonstrate that the magnitude of the resistivity anisotropy in the iron tellurides is correlated with the amount of impurities, implying that the resistivity anisotropy originates from an exotic impurity effect like that in the iron arsenides. This suggests that the anisotropic carrier scattering by impurities is a universal phenomenon in the magneto-structurally ordered phase of the iron-based materials.",1501.00774v1 2015-05-21,Resistance minimum and electrical conduction mechanism in polycrystalline CoFeB thin films,"The temperature dependent resistance $R$($T$) of polycrystalline ferromagnetic CoFeB thin films of varying thickness are analyzed considering various electrical scattering processes. We observe a resistance minimum in $R$($T$) curves below $\simeq$ 29 K, which can be explained as an effect of intergranular Coulomb interaction in a granular system. The structural and Coulomb interaction related scattering processes contribute more as the film thickness decreases implying the role of disorder and granularity. Although the magnetic contribution to the resistance is the weakest compared to these two, it is the only thickness independent process. On the contrary, the negative coefficient of resistance can be explained by electron interaction effect in disordered amorphous films.",1505.05711v2 2015-10-29,Magneto-transport behaviour of Bi2Se3-xTex: Role of disorder,"Magnetoresistance and Hall resistance measurements have been carried out in fastcooled single crystals of Bi2Se3-xTex (x: 0 to 2) in 4 to 300 K temperature range, under magnetic fields up to 15 T. The variation of resistivity with temperature that points to a metallic behaviour in Bi2Se3, shows an upturn at low temperatures in the Te doped samples. Magnetoresistance measurements in Bi2Se3 show clear signatures of Shubnikov de Hass oscillations that gets suppressed in the Te doped samples. In the Bi2SeTe2 sample, the magneto-resistance shows a cusp like positive magneto-resistance at low magnetic fields and low temperatures, a feature associated with weak antilocalisation (WAL), that crosses over to negative magneto-resistance at higher fields. The qualitatively different magnetotransport behaviour seen in Bi2SeTe2 as compared to Bi2Se3 is rationalised in terms of the disorder, through an estimate of the carrier density, carrier mobility and an analysis in terms of the Ioffe Regel criterion with support from Hall Effect measurements.",1510.08561v1 2015-12-10,Mini array of quantum Hall devices based on epitaxial graphene,"Series connection of four quantum Hall effect (QHE) devices based on epitaxial graphene films was studied for realization of a quantum resistance standard with an up-scaled value. The tested devices showed quantum Hall plateaux RH,2 at filling factor i = 2 starting from relatively low magnetic field (between 4 T and 5 T) when temperature was 1.5 K. Precision measurements of quantized Hall resistance of four QHE devices connected by triple series connections and external bonding wires were done at B = 7 T and T = 1.5 K using a commercial precision resistance bridge with 50 microA current through the QHE device. The results showed that the deviation of the quantized Hall resistance of the series connection of four graphene-based QHE devices from the expected value of 4*RH,2 = 2h/e^2 was smaller than the relative standard uncertainty of the measurement (< 1*10^-7) limited by the used resistance bridge.",1512.03163v2 2016-01-04,Making Consistent Contacts to Graphene: Effect of Architecture and Growth Induced Defects,"The effect of contact architecture, graphene defect density and metal-semiconductor work function difference on resistivity of metal-graphene contacts have been investigated. An architecture with metal on the bottom of graphene is found to yield resistivities that are lower, by a factor of 4, and most consistent as compared to metal on top of graphene. Growth defects in graphene film were found to further reduce resistivity by a factor of 2. Using a combination of method and metal used, the contact resistivity of graphene has been decreased by a factor of 10 to 1200 +- 250 Ohm-um using Palladium as the contact metal. While the improved consistency is due to the metal being able to contact uncontaminanted graphene in the metal on the bottom architecture, lower contact resistivities observed on defective graphene with the same metal is attributed to the increased number of modes of quantum transport in the channel.",1601.00429v1 2016-06-13,Effect of interstitial impurities on the field dependent microwave surface resistance of niobium,"Previous work has demonstrated that the radio frequency surface resistance of niobium resonators is dramatically reduced when nitrogen impurities are dissolved as interstitial in the material. The origin of this effect is attributed to the lowering of the Mattis and Bardeen surface resistance contribution with increasing accelerating field. Meanwhile, an enhancement of the sensitivity to trapped magnetic field is typically observed for such cavities. In this paper we conduct the first systematic study on these different components contributing to the total surface resistance as a function of different levels of dissolved nitrogen, in comparison with standard surface treatments for niobium resonators. Adding these results together we are able to show for the first time which is the optimum surface treatment that maximizes the Q-factor of superconducting niobium resonators as a function of expected trapped magnetic field in the cavity walls. These results also provide new insights on the physics behind the change in the field dependence of the Mattis and Bardeen surface resistance, and of the trapped magnetic vortex induced losses in superconducting niobium resonators.",1606.04174v1 2016-10-18,Dichotomy between in-plane magnetic susceptibility and resistivity anisotropies in extremely strained $BaFe_{2}As_{2}$,"The in-plane resistivity and uniform magnetic susceptibility anisotropies of $BaFe_{2}As_{2}$ are obtained with a new method, in which a large symmetry-breaking uniaxial strain is applied using a substrate with a very anisotropic thermal expansion. The resistivity anisotropy and its corresponding elastoresistivity exhibit very similar diverging behavior as those obtained from piezo-stack experiments. This suggests that the resistivity anisotropy is more a direct measure of magnetism than of nematicity, since the nematic transition is no longer well-defined under a large strain. In strong contrast to the large resistivity anisotropy above $T_{N}$, the anisotropy of the in-plane magnetic susceptibility develops largely below $T_{N}$. Using an itinerant model, we show that the observed anisotropy ($\chi_{b}>\chi_{a}$) is determined by spin-orbit coupling and the orientation of the magnetic moments in the antiferromagnetic phase, and that the anisotropy is dominated by intra-orbital ($yz,yz$) contributions of the Umklapp susceptibility.",1610.05575v2 2016-12-15,Reaction-Drift Model for Switching Transients in Pr$_{0.7}$Ca$_{0.3}$MnO$_3$ Based Resistive RAM,"Earlier, the DC hole-current modeling of PCMO RRAM by drift-diffusion (DD) including self-heating (SH) in TCAD (but without ionic transport) was able to explain the experimentally observed SCLC characteristics, prior to resistive switching. Further, transient analysis using DD+SH model was able to reproduce the experimentally observed fast current increase at ~100ns timescale followed by saturation increases, prior to resistive switching. However, resistive switching requires the inclusion of ionic transport. We propose a Reaction-Drift (RD) model of oxide ions, which is combined with the DD+SH model. Experimentally, SET operations consist of 3 stages and RESET operations consists of 4 stages. The DD+SH+RD model is able to reproduce the entire transient behavior over 10$^{-8}$-1s range in timescale for both SET and RESET operations for a range of bias, temperature. Remarkably, a universal RESET behaviour of $log(I)\propto m*log(t)$, where $m\approx -1/10$, is reproduced. The quantitatively different voltage time dilemma for SET and RESET is also replicated for a range of ambient temperature. This demonstrates a comprehensive model for resistance switching in PCMO based RRAM.",1612.05293v2 2018-06-20,Domain wall resistance in CoFeB-based heterostructures with interface Dzyaloshinskii-Moriya interaction,"We have studied the domain wall resistance in W/Ta/CoFeB/MgO heterostructures. The Ta layer thickness is varied to control the type of domain walls via changes in the interfacial Dzyaloshinskii Moriya interaction. We find a nearly constant domain wall resistance against the Ta layer thickness. Adding contributions from the anisotropic magnetoresistance, spin Hall magnetoresistance and anomalous Hall effect describe well the domain wall resistance of the thick Ta layer films. However, a discrepancy remains for the thin Ta layer films wherein chiral N\'eel-like domain walls are found. These results show the difficulty of studying the domain wall type from resistance measurements.",1806.07750v1 2019-02-12,Designing multi-level resistance states for multi-bit storage using half doped manganites,"Designing nonvolatile multi-level resistive devices is the necessity of time to go beyond traditional one-bit storage systems, thus enhancing the storage density. Here, we explore the electronic phase competition scenario to design multi-level resistance states using a half doped CE-type charge ordered insulating bulk manganite, $Sm_{0.5}Ca_{0.25}Sr_{0.25}MnO_3$ (SCSMO). By introducing electronic phase coexistence in a controllable manner in SCSMO, we show that the system can be stabilized into several metastable states, against thermal cycling, up to 62 K. As a result the magnetization (and the resistivity) remains unaltered during the thermal cycling. Monte Carlo calculations using two-band double exchange model, including super-exchange, electron-phonon coupling, and quenched disorder, show that the system freezes into a phase coexistence metastable state during the thermal cycling due to the chemical disorder in SCSMO. Using the obtained insights we outline a pathway by utilizing four reversible metastable resistance states to design a prototype multi-bit memory device.",1902.04377v1 2019-03-02,On the origin of the anomalous peak in the resistivity of TiSe$_2$,"Resistivity measurements of TiSe$_2$ typically show only a weak change in gradient at the charge density wave transition at $T_{CDW}\approx$ 200~K, but more prominently feature a broad peak at a lower $T_{peak}\sim$ 165~K, which has remained poorly understood despite decades of research on the material. Here we present quantitative simulations of the resistivity using a simplified parametrization of the normal state band structure, based on recent photoemission data. Our simulations reproduce the overall profile of the resistivity of TiSe$_2$, including its prominent peak, without implementing the CDW at all. We find that the peak in resistivity corresponds to a crossover between a low temperature regime with electron-like carriers only, to a regime around room temperature where thermally activated and highly mobile hole-like carriers dominate the conductivity. Even when implementing substantial modifications to model the CDW below the transition temperature, we find that these thermal population effects still dominate the transport properties of TiSe$_2$.",1903.00756v1 2012-06-13,Modelling of Current Percolation Channels in Emerging Resistive Switching Elements,"Metallic oxides encased within Metal-Insulator-Metal (MIM) structures can demonstrate both unipolar and bipolar switching mechanisms, rendering them the capability to exhibit a multitude of resistive states and ultimately function as memory elements. Identifying the vital physical mechanisms behind resistive switching can enable these devices to be utilized more efficiently, reliably and in the long-term. In this paper, we present a new approach for analysing resistive switching by modelling the active core of two terminal devices as 2D and 3D grid circuit breaker networks. This model is employed to demonstrate that substantial resistive switching can only be supported by the formation of continuous current percolation channels, while multi-state capacity is ascribed to the establishment and annihilation of multiple channels.",1206.2746v1 2019-06-07,Extended Nyquist formula for a resistance subject to a heat flow,"The Nyquist formula quantifies the thermal noise driven fluctuations of voltage across a resistance in equilibrium. We deal here with the case of a resistance driven out of equilibrium by putting it in contact with two thermostats at different temperatures. We reach a non-equilibrium steady state where a heat flux is flowing through the resistance. Our measurements demonstrate anyway that a simple extension of the Nyquist formula to the non uniform temperature field describes with an excellent precision the thermal noise. For a metallic ohmic material, the fluctuations are actually equivalent to those of a resistance in equilibrium with a single thermostat at the mean temperature between the hot and cold sources.",1906.02974v2 2020-06-22,Optimal design of a bilayer for the highest thermal resistance: A lesson learned from the shells of snails from hydrothermal extreme environment,"Inspired by the unique design of the shells of snails inhabiting the deep-sea hydrothermal environment, here we theoretically study the temperature response of a bilayer to an external thermal impulse. A semi-analytical solution to the temperature field in the bilayer is obtained, allowing us to assess the peak temperature that occurs on the inner wall as a quantitative indicator of the thermal resistance of the bilayer. The structural determining factors of the thermal resistance of a bilayer are then investigated by examining the effects of the stacking sequence and volume fractions of the constitutive layers on the peak temperature on the inner wall. Our results indicate that the stacking sequence of the two layers in a bilayer, as well as their volume fractions, play important roles in determining the thermal resistance. For two layers with given materials, there exists an optimal stacking sequence and thickness ratio giving rise to the best thermal resistance. The results of our work not only account for the unique laminated design of the snail shells from hydrothermal environments but also provide practical guidelines for the design of multilayer thermal barriers in engineering.",2006.11987v1 2020-11-01,Reduction of interfacial thermal resistance of overlapped graphene by bonding carbon chains,"Exploring the mechanism of interfacial thermal transport and reducing the interfacial thermal resistance is of great importance for thermal management and modulation. Herein, the interfacial thermal resistance between overlapped graphene nanoribbons is largely reduced by adding bonded carbon chains by performing molecular dynamics simulations. And the analytical model (cross-interface model, CIM) is utilized to analyze and explain the two-dimensional thermal transport mechanism at cross-interface. An order of magnitude reduction in interfacial thermal resistance is found as the graphene nanoribbons are bonded by just one carbon chain. Interestingly, the decreasing rate of interfacial thermal resistance slows down gradually with the increasing of the number of carbon chains, which can be explained by the proposed theoretical relationship based on CIM. Moreover, by the comparison of CIM and traditional simplified model, the accuracy of CIM is verified and demonstrated in overlapped graphene nanoribbons. This work provides a new way to improve the interfacial thermal transport and reveal the essential mechanism for low-dimensional materials applied in thermal management.",2011.00494v1 2021-04-15,Origins of anisotropic transport in electrically-switchable antiferromagnet $\mathrm{Fe_1/3NbS_2}$,"Recent experiments on the antiferromagnetic intercalated transition metal dichalcogenide $\mathrm{Fe_{1/3}NbS_2}$ have demonstrated reversible resistivity switching by application of orthogonal current pulses below its magnetic ordering temperature, making $\mathrm{Fe_{1/3}NbS_2}$ promising for spintronics applications. Here, we perform density functional theory calculations with Hubbard U corrections of the magnetic order, electronic structure, and transport properties of crystalline $\mathrm{Fe_{1/3}NbS_2}$, clarifying the origin of the different resistance states. The two experimentally proposed antiferromagnetic ground states, corresponding to in-plane stripe and zigzag ordering, are computed to be nearly degenerate. In-plane cross sections of the calculated Fermi surfaces are anisotropic for both magnetic orderings, with the degree of anisotropy sensitive to the Hubbard U value. The in-plane resistance, computed within the Kubo linear response formalism using a constant relaxation time approximation, is also anisotropic, supporting a hypothesis that the current-induced resistance changes are due to a repopulating of AFM domains. Our calculations indicate that the transport anisotropy of $\mathrm{Fe_{1/3}NbS_2}$ in the zigzag phase is reduced relative to stripe, consistent with the relative magnitudes of resistivity changes in experiment. Finally, our calculations reveal the likely directionality of the current-domain response, specifically, which domains are energetically stabilized for a given current direction.",2104.07591v1 2021-08-01,First-principles study on the electrical resistivity in zirconium dichalcogenides with multi-valley bands: mode-resolved analysis of electron-phonon scattering,"Based on the first-principles calculations, we study the electron-phonon scattering effect on the resistivity in the zirconium dichalcogenides, $\text{Zr}_{}\text{S}_{2}$ and $\text{Zr}_{}\text{Se}_{2}$, whose electronic band structures possess multiple valleys at conduction band minimum. The computed resistivity exhibits non-linear temperature dependence, especially for $\text{Zr}_{}\text{S}_{2}$, which is also experimentally observed on some TMDCs such as $\text{Ti}_{}\text{S}_{2}$ and $\text{Zr}_{}\text{Se}_{2}$. By performing the decomposition of the contributions of scattering processes, we find that the intra-valley scattering by acoustic phonons mainly contributes to the resistivity around 50 K. Moreover, the contribution of the intra-valley scattering by optical phonons becomes dominant even above 80 K, which is a sufficiently low temperature compared with their frequencies. By contrast, the effect of the inter-valley scattering is found to be not significant. Our study identifies the characteristic scattering channels in the resistivity of the zirconium dichalcogenides, which provides critical knowledge to microscopically understand electron transport in systems with multi-valley band structure.",2108.00474v1 2024-02-15,What can we learn from nonequilibrium response of a strange metal?,"We critically address the recent experiment [Science 382, 907 (2023)] on nonequilibrium transport and noise in a strange metal YbRh2Si2 patterned into the nanowire shape. In the long device, resistivity, differential resistance and current noise data seem to be consistent allowing us to extract electron-phonon coupling and the temperature dependence of electron-phonon scattering length. The obtained values can be reconciled with the experimental data for the short device only assuming the significant contact resistance. We discuss its possible origin as due to the current redistribution between YbRh2Si2 and its gold covering, and reveal that this redistribution contact resistance should be proportional to the YbRh2Si2 resistivity. We also discuss some subtleties of the noise measurements. Overall, neglecting electron-phonon energy relaxation even in the shortest devices is arguable so that the observed shot noise suppression can hardly be attributed to the failure of quasiparticle concept.",2402.09946v1 2023-07-27,Reduced stress propagation leads to increased mechanical failure resistance in auxetic materials,"Materials with negative Poisson ratio have the counter-intuitive property of expanding laterally when they are stretched longitudinally. They are accordingly termed auxetic, from the Greek auxesis meaning to increase. Experimental studies have demonstrated auxetic materials to have superior material properties, compared with conventional ones. These include synclastic curvature, increased acoustic absorption, increased resilience to material fatigue, and increased resistance to mechanical failure. Until now, the latter observations have remained poorly understood theoretically. With this motivation, the contributions of this work are twofold. First, we elucidate analytically the way in which stress propagates spatially across a material following a localised plastic failure event, finding a significantly reduced stress propagation in auxetic materials compared with conventional ones. In this way, a plastic failure event occurring in one part of a material has a reduced tendency to trigger knock-on plastic events in neighbouring regions. Second, via the numerical simulation of a lattice elastoplastic model, we demonstrate a key consequence of this reduced stress propagation to be an increased resistance to mechanical failure. This is seen not only via an increase in the externally measured yield strain, but also via a decreased tendency for plastic damage to percolate internally across a sample in catastrophic system-spanning clusters.",2307.14914v2 2014-11-28,Signature of high Tc around 25K in higher quality heavily boron-doped diamond,"Diamond has outstanding physical properties: the hardest known material, a wide band gap, the highest thermal conductivity, and a very high Debye temperature. In 2004, Ekimov et al. discovered that heavily boron-doped (B-doped) diamond becomes a superconductor around 4 K. Our group successfully controlled the boron concentration and synthesized homoepitaxially grown superconducting diamond films by a CVD method. By CVD method, we found that superconductivity appears when the boron concentration (nB) exceeds a metal-insulator transition concentration of 3.0x10^20 cm^-3 and its Tczero increases up to 7.4 K with increasing nB. We additionally elucidated that the holes formed at the valence band are responsible for the metallic states leading to superconductivity. The calculations predicted that the hole doping into the valence band induces strong attractive interaction and a rapid increase in Tc with increasing boron concentration. According to the calculations, if substitutional doped boron could be arranged periodically or the degree of disorder is reduced, a Tc of approximately 100 K could be achieved via minimal percent doping. In this work, we have successfully observed zero resistivity above 10 K and an onset of resistivity reduction at 25.2 K in heavily B-doped diamond film. However, the effective carrier concentration is similar to that of superconducting diamond with a lower Tc. We found that the carrier has a longer mean free path and lifetime than previously reported, indicating that this highest Tc diamond has better crystallinity compared to that of other superconducting diamond films. In addition, the susceptibility shows a small transition above 20 K in the high quality diamond, suggesting a signature of superconductivity above 20 K. These results strongly suggest that heavier carrier doped defect-free crystalline diamond could give rise to high Tc diamond.",1411.7752v1 2019-08-21,Fatigue-resistant high-performance elastocaloric materials via additive manufacturing,"Elastocaloric cooling, which exploits the latent heat released and absorbed as stress-induced phase transformations are reversibly cycled in shape memory alloys, has recently emerged as a frontrunner in non-vapor-compression cooling technologies. The intrinsically high thermodynamic efficiency of elastocaloric materials is limited only by work hysteresis. Here, we report on creating high-performance low-hysteresis elastocaloric cooling materials via additive manufacturing of Titanium-Nickel (Ti-Ni) alloys. Contrary to established knowledge of the physical metallurgy of Ti-Ni alloys, intermetallic phases are found to be beneficial to elastocaloric performances when they are combined with the binary Ti-Ni compound in nanocomposite configurations. The resulting microstructure gives rise to quasi-linear stress-strain behaviors with extremely small hysteresis, leading to enhancement in the materials efficiency by a factor of five. Furthermore, despite being composed of more than 50% intermetallic phases, the reversible, repeatable elastocaloric performance of this material is shown to be stable over one million cycles. This result opens the door for direct implementation of additive manufacturing to elastocaloric cooling systems where versatile design strategy enables both topology optimization of heat exchangers as well as unique microstructural control of metallic refrigerants.",1908.07900v1 2019-07-31,Quantum oscillations in diamond field effect transistors with a h-BN gate dielectric,"Diamond has attracted attention as a next-generation semiconductor because of its various exceptional properties such as a wide bandgap and high breakdown electric field. Diamond field effect transistors, for example, have been extensively investigated for high-power and high-frequency electronic applications. The quality of their charge transport (i.e., mobility), however, has been limited due to charged impurities near the diamond surface. Here, we fabricate diamond field effect transistors by using a monocrystalline hexagonal boron nitride as a gate dielectric. The resulting high mobility of charge carriers allows us to observe quantum oscillations in both the longitudinal and Hall resistivities. The oscillations provide important information on the fundamental properties of the charge carriers, such as effective mass, lifetime, and dimensionality. Our results indicate the presence of a high-quality two-dimensional hole gas at the diamond surface and thus pave the way for studies of quantum transport in diamond and the development of low-loss and high-speed devices.",1907.13500v2 2021-12-08,High-Mg Calcite Nanoparticles Within a Low-Mg Calcite Matrix via Spinodal Decomposition: A Widespread Phenomenon in Biomineralization,"During the process of biomineralization, organisms utilize various biostrategies to enhance the mechanical durability of their skeletons. In this work, we establish that the presence of high-Mg nanoparticles embedded within lower Mg calcite matrices is a widespread strategy utilized by various organisms from different kingdoms and phyla to improve the mechanical properties of their high Mg calcite skeletons. We show that such phase separation and the formation of high-Mg nanoparticles are achieved through spinodal decomposition of an amorphous Mg calcite precursor. Such decomposition is independent of the biological characteristics of the studied organisms belonging to different phyla and even kingdoms, but rather originates from their similar chemical composition and a specific Mg content within their skeletons, which generally ranges from 14 to 48 mol percent of Mg. We show evidence of high Mg calcite nanoparticles in the cases of 6 biologically different organisms all demonstrating more than 14 mol percent Mg calcite, and consider it likely that this phenomenon is immeasurably more prevalent in nature. We also establish the absence of these high Mg nanoparticles in organisms whose Mg content is lower than 14 mol percent, providing further evidence that whether or not spinodal decomposition of an amorphous Mg calcite precursor takes place is determined by the amount of Mg it contains. The valuable knowledge gained from this biostrategy significantly impacts the understanding of how biominerals, though comprised of intrinsically brittle materials, can effectively resist fracture.",2112.04141v1 2022-08-11,Superconductivity above 80 K in polyhydrides of hafnium,"Studies on polyhydrides are attracting growing attentions recently due to their potential high temperature superconductivity (SC). We here report the discovery of SC in hafnium polyhydrides at high pressures. The hafnium superhydrides are synthesized at high pressure and high temperature conditions using diamond anvil cell in combination with in-situ high pressure laser heating technique. The SC was investigated by in-situ high pressure resistance measurements in applied magnetic fields. A superconducting transition with onset Tc ~83 K was observed at 243 GPa. The upper critical field Hc2(0) was estimated to be 24 Tesla by GL theory and the consequent superconducting coherent length to be ~37 angstrom. Our results suggest that the superconducting phase is from C2/m-HfH14. This is the first 5d transition metal polyhydride superconductor with Tc above the liquid nitrogen temperature.",2208.05816v2 2001-05-16,Superconducting properties of well-shaped MgB2 single crystal,"We report measurements of the transport and the magnetic properties of high-quality, sub-millimeter-sized MgB2 single crystals with clear hexagonal-plate shapes. The low-field magnetization and the magnetic hysteresis curves show the vortex pinning of these crystals to be very weak. The Debye temperature of $\Theta_{D}\sim 1100$ K, obtained from the zero-field resistance curve, suggests that the normal-state transport properties are dominated by electron-phonon interactions. The resistivity ratio between 40 K and 300 K was about 5, and the upper critical field anisotropy ratio was 3 $\pm$ 0.2 at temperatures around 32 K.",0105330v7 2003-09-24,Quantum Effects in Thermal Conductivity of Solid Krypton - Methane Solutions,"The dynamic interaction of a quantum rotor with its crystalline environment has been studied by measurement of the thermal conductivity of solid Kr1_c(CH4)_c solutions at c = 0.05-0.75 in the temperature region from 2 up to 40K. The thermal resistance of the solutions was mainly determined by the resonance scattering of phonons by CH4 molecules with the nuclear spin I=1 (the nuclear spin of T-species). The influence of the nuclear spin conversion on the temperature dependence of the thermal conductivity k(T) was found: a clearly defined minimum on k(T), its temperature position depending on the CH4 concentration. It was shown that the anisotropy molecular field not increase monotonously with the CH4 concentration. A compensation effect in the mutual orientation arrangement of the neighboring rotors is observed at c > 0.5. The temperature dependence of Kr1_c(CH4)_c is described within the Debye model of thermal conductivity taking into account the lower limit of the phonon mean free path. The anomalous temperature dependence of the thermal resistance shows the evolution of the phonon-rotation coupling at varying temperature. It increases strongly when the character of CH4 rotation changes from the quantum at low temperatures to classical at high temperatures. Also, a jump of thermal conductivity (a sharp increase in k(T) within a narrow temperature range) was observed, whose position varies from 9.7 K to 8.4 K when the CH4 concentration changes from 0.25 to 0.45.",0309542v1 2005-05-19,Strongly correlated properties of the thermoelectric cobalt oxide Ca3Co4O9,"We have performed both in-plane resistivity, Hall effect and specific heat measurements on the thermoelectric cobalt oxide Ca$_{3}$Co$_{4}$O$_{9}$. Four distinct transport regimes are found as a function of temperature, corresponding to a low temperature insulating one up to $T_{min}\approx $63 K, a strongly correlated Fermi liquid up to $T^*\approx $140 K, with $\rho=\rho_0+AT^2$ and $A\approx 3.63$ $10^{-2} \mu \Omega cm/K^{2}$, followed by an incoherent metal with $k_Fl\leq 1$ and a high temperature insulator above T$^{**}\approx $510 K . Specific heat Sommerfeld coefficient $\gamma = 93$ mJ/(mol.K$^{2}$) confirms a rather large value of the electronic effective mass and fulfils the Kadowaki-Woods ratio $A/\gamma^2 \approx 0.45$ 10$^{-5}$ $\mu \Omega cm.K^2/(mJ^2mol^{-2})$. Resistivity measurements under pressure reveal a decrease of the Fermi liquid transport coefficient A with an increase of $T^*$ as a function of pressure while the product $A(T^*)^2/a$ remains constant and of order $h/e^2$. Both thermodynamic and transport properties suggest a strong renormalization of the quasiparticles coherence scale of order $T^*$ that seems to govern also thermopower.",0505464v1 2005-10-03,New Misfit-Layered Cobalt Oxide (CaOH)1.14CoO2,"We found a new cobalt oxide (CaOH)1.14CoO2 by utilizing the high-pressure technique. X-ray and electron diffraction studies revealed that the compound has layer structure which consists of CdI2-type CoO2 layers and rock-salt-type double CaOH atomic layers. The two subcells have incommensurate periodicity along the a-axis, resulting in modulated crystal structure due to the inter-subcell interaction. The structural modulation affects carrier conduction through the potential randomness. We found that the two-dimensional (2-D) variable-range hopping (VRH) regime with hole conduction is dominant at low temperature for this compound, and that the conduction mechanism undergoes crossover from the 2-D VRH regime to thermal activation-energy type one with increasing temperature. Based on the experimental results of resistivity, thermoelectric power, magnetic susceptibility and specific heat measurements, we suggested a possible electronic-band structure model to explain these results. The cobalt t2g-derivative band crosses Fermi energy level near the band edge, yielding small finite density of localized states at the Fermi level in the band. The observed resistivity, Seebeck coefficient, large Pauli paramagnetic component in the magnetic susceptibility and comparatively small Sommerfeld constant in the specific heat are principally attributed to the holes in the t2g-derivative band. We estimated the Wilson ratio to be about 2.8, suggesting the strong electron correlation realized in this compound.",0510031v1 2007-09-12,The Hot-Spot Phenomenon and its Countermeasures in Bipolar Power Transistors by Analytical Electro-Thermal Simulation,"This communication deals with a theoretical study of the hot spot onset (HSO) in cellular bipolar power transistors. This well-known phenomenon consists of a current crowding within few cells occurring for high power conditions, which significantly decreases the forward safe operating area (FSOA) of the device. The study was performed on a virtual sample by means of a fast, fully analytical electro-thermal simulator operating in the steady state regime and under the condition of imposed input base current. The purpose was to study the dependence of the phenomenon on several thermal and geometrical factors and to test suitable countermeasures able to impinge this phenomenon at higher biases or to completely eliminate it. The power threshold of HSO and its localization within the silicon die were observed as a function of the electrical bias conditions as for instance the collector voltage, the equivalent thermal resistance of the assembling structure underlying the silicon die, the value of the ballasting resistances purposely added in the emitter metal interconnections and the thickness of the copper heat spreader placed on the die top just to the aim of making more uniform the temperature of the silicon surface.",0709.1831v1 2007-09-14,An inhomogeneous Josephson phase in thin-film and High-Tc superconductors,"In many cases inhomogeneities are known to exist near the metal (or superconductor)-insulator transition, as follows from well-known domain-wall arguments. If the conducting regions are large enough (i.e. when the T=0 superconducting gap is much larger than the single-electron level spacing), and if they have superconducting correlations, it becomes energetically favorable for the system to go into a Josephson-coupled zero-resistance state before (i.e. at higher resistance than) becoming a ""real"" metal. We show that this is plausible by a simple comparison of the relevant coupling constants. For small grains in the above sense, the electronic grain structure is washed out by delocalization and thus becomes irrelevant. When the proposed ""Josephson state"" is quenched by a magnetic field, an insulating, rather then a metallic, state should appear. This has been shown to be consistent with the existing data on oxide materials as well as ultra-thin films. We discuss the Uemura correlations versus the Homes law, and derive the former for the large-grain Josephson array (inhomogenous superconductor) model. The small-grain case behaves like a dirty homogenous metal. It should obey the Homes law provided that the system is in the dirty supeconductivity limit. A speculation why that is typically the case for d-wave superconductors is presented.",0709.2321v1 2009-03-18,Two-dimensional electrochemical model for mixed conductors: a study of ceria,"A two-dimensional small bias model has been developed for a patterned metal current collector $|$ mixed oxygen ion and electronic conductor (MIEC) $|$ patterned metal current collector electrochemical cell in a symmetric gas environment. Specifically, we compute the electrochemical potential distributions of oxygen vacancies and electrons in the bulk and near the surface for $\text{Pt} | \text{Sm}_{0.15}\text{Ce}_{0.85}\text{O}_{1.925} | \text{Pt}$ symmetric cell in a $\text{H}_2-\text{H}_2\text{O}-\text{Ar}$ (reducing) atmosphere from 500 to $650^o C$. Using a two-dimensional finite-element model, we show that two types of electronic current exist within the cell: an in-plane drift-diffusion current that flows between the gas $|$ ceria chemical reaction site and the metal current collector, and a cross-plane current that flows between the two metal electrodes on the opposite side of the cell. By fitting the surface reaction constant $\tilde k_f^0$ to experimental electrode resistance values while fixing material properties such as bulk ionic and electronic equilibrium defect concentrations and mobilities, we are able to separate the electrode polarization into the surface reaction component and the in-plane electron drift-diffusion component. We show that for mixed conductors with a low electronic conductivity (a function of oxygen partial pressure) or a high surface reaction rate constant, the in-plane electron drift-diffusion resistance can become rate-limiting in the electrode reaction.",0903.3250v1 2009-11-11,The pseudogap behavior in the stoichiometric FeSe superconductor (Tc~9.4 K),"This paper reports the synthesis and superconducting behaviors of the tetragonal iron-chalcogenide superconductor FeSe. The electrical resistivity and magnetic moment measurements confirmed its superconductivity with a $T_c^{zero}$ and $T_c^{mag}$ at 9.4 K under ambient pressure. EPMA indicated the sample to have a stoichiometric Fe:Se ratio of 1:1 ($\pm$0.02). The Seebeck coefficient which was 12.3 $\mu$V/K at room temperature, changed to a negative value near 200 K, indicating it to be a two carriers material. Above $T_c$, the $\rho(T)$ curve revealed an 'S' shape. Hence $d\rho(T)/dT$, and $d^2\rho(T)/dT^2$ showed pseudogap-like behavior at $T^*$=110 K according to the resistivity curvature mapping (RCM) method for high $T_c$ cuprates. Moreover, the magnetoresistance $\rho_H(T)/\rho_{H=0}$ under a magnetic field and the Seebeck coefficient $S(T)$ revealed revealed pseudogap-like behavior near $T^*$. Interestingly, at the same temperature, 30 K, the sign of $S(T)$ and all signs of $d^2\rho(T)/dT^2$ changed from negative to positive above $T_c$.",0911.2045v2 2010-07-22,Anisotropic fluctuations and quasiparticle excitations in FeSe_0.5Te_0.5,"We present data for the temperature dependence of the magnetic penetration depth lambda(T), heat capacity C(T), resistivity R(T) and magnetic torque ?tau for highly homogeneous single crystal samples of Fe1:0Se0:44(4)Te0:56(4). lambda(T) was measured down to 200mK in zero field. We find lambda(T) follows a power law lambda~T^n with n = 2.2 +/- 0.1. This is similar to some 122 iron-arsenides and likely results from a sign-changing pairing state combined with strong scattering. Magnetic fields of up to B =55T or 14T were used for the ? tau(B) and C(T)/R(T) measurements respectively. The specific heat, resistivity and torque measurements were used to map out the (H,T) phase diagram in this material. All three measurements were conducted on exactly the same single crystal sample so that the different information revealed by these probes is clearly distinguished. Heat capacity data strongly resemble those found for the high Tc cuprates, where strong fluctuation effects wipe-out the phase transition at Hc2. Unusually, here we find the fluctuation effects appear to be strongly anisotropic.",1007.3914v2 2010-11-09,Frustrated Metastable Behavior of Magnetic and Transport Properties in Charge Ordered La1-xCaxMnO3+d Manganites,"We have studied the effect of metastable, irreversibility induced by repeated thermal cycles on the electric transport and magnetization of polycrystalline samples of La1-xCaxMnO3 (0.48\leq x \leq 0.55) close to charge ordering. With time and thermal cycling (T<300 K) there is an irreversible transformation of the low-temperature phase from a partially ferromagnetic and metallic to one that is less ferromagnetic and highly resistive for the composition close to charge ordering (x=050 and 0.52). Irrespective of the actual ground state of the compound, the effect of thermal cycling is towards an increase of the amount of the insulating phase. We have observed the magnetic relaxation in the metastable state and also the revival of the metastable state (in a relaxed sample) due to high temperature thermal treatment. We observed changes in the resistivity and magnetization as the revived metastable state is cycled. The time changes in the magnetization are logarithmic in general and activation energies are consistent with those expected for electron transfer between Mn ions. Changes induced by thermal cycling can be inhibited by applying magnetic field. These results suggest that oxygen non-stoichiometry results in mechanical strains in this two-phase system, leading to the development of frustrated metastable states which relax towards the more stable charge-ordered and antiferromagnetic microdomains. Our results also suggest that the growth and coexistence of phases gives rise to microstructural tracks and strain accommodation, producing the observed irreversibility.",1011.2179v1 2011-05-17,The metallic transport of (TMTSF)_2X organic conductors close to the superconducting phase,"Comparing resistivity data of quasi-one dimensional superconductors (TMTSF)_2PF_6 and (TMTSF)_2ClO_4 along the least conducting c*-axis and along the high conductivity a -axis as a function of temperature and pressure, a low temperature regime is observed in which a unique scattering time governs transport along both directions of these anisotropic conductors. However, the pressure dependence of the anisotropy implies a large pressure dependence of the interlayer coupling. This is in agreement with the results of first-principles DFT calculations implying methyl group hyperconjugation in the TMTSF molecule. In this low temperature regime, both materials exhibit for rc a temperature dependence aT + bT^2. Taking into account the strong pressure dependence of the anisotropy, the T-linear rc is found to correlate with the suppression of the superconducting Tc, in close analogy with ra data. This work is revealing the domain of existence of the 3D coherent regime in the generic (TMTSF)_2X phase diagram and provides further support for the correlation between T-linear resistivity and superconductivity in non-conventional superconductors.",1105.3323v2 2011-11-29,Towards the Realization of Higher Connectivity in MgB2 Conductors: In-situ or Sintered Ex-situ?,"The two most common types of MgB2 conductor fabrication technique - in-situ and ex-situ - show increasing conflicts concerning the connectivity, an effective current-carrying cross-sectional area. An in-situ reaction yields a strong intergrain coupling with a low packing factor, while an ex-situ process using pre-reacted MgB2 yields tightly packed grains, however, their coupling is much weaker. We studied the normal-state resistivity and microstructure of ex-situ MgB2 bulks synthesized with varied heating conditions under ambient pressure. The samples heated at moderately high temperatures of ~900{\deg}C for a long period showed an increased packing factor, a larger intergrain contact area and a significantly decreased resistivity, all of which indicate the solid-state self-sintering of MgB2. Consequently the connectivity of the sintered ex-situ samples exceeded the typical connectivity range 5-15% of the in-situ samples. Our results show self-sintering develops the superior connectivity potential of ex-situ MgB2, though its intergrain coupling is not yet fulfilled, to provide a strong possibility of twice or even much higher connectivity in optimally sintered ex-situ MgB2 than in in-situ MgB2.",1111.6767v2 2012-07-25,Metallic state in La-doped YBa$_2$Cu$_3$O$_y$ thin films with $n$-type charge carriers,"We report hole and electron doping in La-doped YBa$_2$Cu$_3$O$_y$(YBCO) thin films synthesized by pulsed laser deposition technique and subsequent \emph{in-situ} postannealing in oxygen ambient and vaccum. The $n$-type samples show a metallic behavior below the Mott limit and a high carrier density of $\sim2.8$ $\times$ 10$^{21}$ cm$^{-3}$ at room temperature (\emph{T}) at the optimally reduced condition. The in-plane resistivity ($\rho$$_{ab}$) of the $n$-type samples exhibits a quadratic \emph{T} dependence in the moderate-\emph{T} range and shows an anomaly at a relatively higher \emph{T} probably related to pseudogap formation analogous to underdoped Nd$_{2-x}$Ce$_x$CuO$_4$ (NCCO). Furthermore, $\rho$$_{ab}$(T), \emph{T}$_c$ and \emph{T} with minimum resistivity (\emph{T}$_{min}$) were investigated in both $p$- and $n$-side. The present results reveal the $n$-$p$ asymmetry (symmetry) within the metallic-state region in an underdoped cuprate and suggest the potential toward ambipolar superconductivity in a single YBCO system.",1207.5914v1 2012-11-28,Photoconductivity effects in mixed-phase BSCCO whiskers,"We report on combined photoconductivity and annealing experiments in whisker-like crystals of the Bi-Sr-Ca-Cu-O (BSCCO) high-Tc superconductor. Both single-phase Bi2Sr2CaCu2O8+\delta (Bi-2212) samples and crystals of the mixed phases Bi2Sr2Ca2Cu3O10+x (Bi-2223)/Bi-2212 have been subjected to annealing treatments at 90{\deg}C in air in a few hours steps, up to a maximum total annealing time of 47 h. At every step, samples have been characterized by means of electrical resistance vs temperature (R vs T) and resistance vs time at fixed temperature (R vs t) measurements, both in the dark and under illumination with a UV-VIS halogen arc lamp. A careful comparison of the results from the two techniques has shown that, while for single-phase samples no effect is recorded, for mixed-phase samples an enhancement in the conductivity that increases with increasing the annealing time is induced by the light at the nominal temperature T = 100 K, i.e. at an intermediate temperature between the critical temperatures of the two phases. A simple pseudo-1D model based on the Kudinov's scheme [Kudinov et al., Phys. Rev. B 47, 9017-28, (1993)] has been developed to account for the observed effects, which is based on the existence of Bi-2223 filaments embedded in the Bi-2212 matrix and on the presence of electronically active defects at their interfaces. This model reproduces fairly well the photoconductive experimental results and shows that the length of the Bi-2223 filaments decreases and the number of defects increases with increasing the annealing time.",1211.6594v1 2013-01-03,Studies of YBa2Cu3O6+x degradation and surface conductivity properties by Scanning Spreading Resistance Microscopy,"Local surface conductivity properties and surface degradation of c-axis oriented YBa2Cu3O6+x (YBCO) thin films were studied by Scanning Spreading Resistance Microscopy (SSRM). For the surface degradation studies, the YBCO surface was cleaned by ion beam etching and the SSRM surface conductivity map has been subsequently repeatedly measured over several hours in air and pure nitrogen. Average surface conductivity of the scanned area was gradually decreasing over time in both cases, faster in air. This was explained by oxygen out-diffusion in both cases and chemical reactions with water vapor in air. The obtained surface conductivity images also revealed its high inhomogenity on micrometer and nanometer scale with numerous regions of highly enhanced conductivity compared to the surroundings. Furthermore, it has been shown that the size of these conductive regions considerably depends on the applied voltage. We propose that such inhomogeneous surface conductivity is most likely caused by varying thickness of degraded YBCO surface layer as well as varying oxygen concentration (x parameter) within this layer, what was confirmed by scanning Auger electron microscopy (SAM). In our opinion the presented findings might be important for analysis of current-voltage and differential characteristics measured on classical planar junctions on YBCO as well as other perovskites.",1301.0397v1 2013-02-21,Electronic transport on carbon nanotube networks: a multiscale computational approach,"Carbon nanotube networks are one of the candidate materials to function as malleable, transparent, conducting films, with the technologically promising application of being used as flexible electronic displays. Nanotubes disorderly distributed in a film offers many possible paths for charge carriers to travel across the entire system, but the theoretical description of how this charge transport occurs is rather challenging for involving a combination of intrinsic nanotube properties with network morphology aspects. Here we attempt to describe the transport properties of such films in two different length scales. Firstly, from a purely macroscopic point of view we carry out a geometrical analysis that shows how the network connectivity depends on the nanotube concentration and on their respective aspect ratio. Once this is done, we are able to calculate the resistivity of a heavily disordered networked film. Comparison with experiment offers us a way to infer about the junction resistance between neighbouring nanotubes. Furthermore, in order to guide the frantic search for high-conductivity films of nanotube networks, we turn to the microscopic scale where we have developed a computationally efficient way for calculating the ballistic transport across these networks. While the ballistic transport is probably not capable of describing the observed transport properties of these films, it is undoubtedly useful in establishing an upper value for their conductivity. This can serve as a guideline in how much room there is for improving the conductivity of such networks.",1302.5379v1 2013-12-05,Giant topological Hall effect in strained Fe$_{0.7}$Co$_{0.3}$Si epilayers,"The coupling of electron spin to real-space magnetic textures leads to a variety of interesting magnetotransport effects. The skyrmionic spin textures often found in chiral B20-lattice magnets give rise, via real-space Berry phases, to the topological Hall effect, but it is typically rather small. Here, B20-ordered Fe$_{0.7}$Co$_{0.3}$Si epilayers display a giant topological Hall effect due to the combination of three favourable properties: they have a high spin-polarisation, a large ordinary Hall coefficient, and dense chiral spin textures. The topological Hall resistivity is as large as 820 n$\Omega$cm at helium temperatures. Moreover, we observed a drop in the longitudinal resistivity of 100 n$\Omega$cm at low temperatures in the same field range, suggesting that it is also of topological origin. That such strong effects can be found in material grown in thin film form on commercial silicon wafer bodes well for skyrmion-based spintronics.",1312.1722v1 2013-12-23,Signatures of electronic phase separation in the Hall effect of anisotropically strained La0.67Ca0.33MnO3 films,"Systematic transport measurements have been performed on a series of La0.67Ca0.33MnO3 (LCMO) thin films with varying degrees of anisotropic strain. The strain is induced via epitaxial growth on NdGaO3(001) substrates and varied by controlling the thermal annealing time. An antiferromagnetic insulating (AFI) state, possibly associated with charge ordering, emerges upon thermal annealing. The Hall effect in these materials exhibits features that are indicative of a percolative phase transition and correlate closely with the emergence of the AFI state. In the paramagnetic phase, the Hall resistivity takes on two slopes in all samples: a decreasing negative slope with increasing temperature at low fields, which is attributed to the carrier hopping motion, and an almost temperature independent positive slope at high fields due to diffusive transport of holes. Significantly, the crossover fields of the Hall resistivity slope at different temperatures correspond to the same magnetization, which is interpreted as the critical point of a magnetic field-driven percolative phase transition. At lower temperatures near the zero-field metal-insulator transition, pronounced enhancement of the Hall coefficient with the development of the AFI state is observed. The enhancement peaks near the magnetic field-driven percolation; its magnitude correlates with the strength of the AFI state and is suppressed with the melting of the AFI state by an in-plane magnetic field. The observations resemble many features of the enhancement of the Hall coefficient in granular metal films near the composition-driven percolation.",1312.6670v1 2014-04-16,Origin of High Temperature Oxidation Resistance of Ti-Al-Ta-N Coatings,"Alloying Ti-Al-N coatings with Ta has proven to enhance their hardness, thermal stability, and oxidation resistance. However, especially for arc-evaporated Ti-Al-Ta-N coatings only limited information on the detailed influence of the elements on various properties is available. Therefore, we have developed arc-evaporated Ti1-x-yAlxTayN coatings with various Al (x = 0.50 - 0.65) and Ta (y = 0.00 - 0.15) contents. While the thermal stability of our coatings during annealing in inert He atmosphere increases with increasing Ta content, best results are obtained for specific Ta-Al ratios during oxidation. Single phase cubic Ti0.32Al0.60Ta0.08N yields a mass-gain of only ~5 % after 5 h at 950 {\deg}C in synthetic air, whereas Ti0.35Al0.65N is completely oxidized after 15 min. This is in part based on the suppressed anatase and direct rutile TiO2 formation at a defined Ta-Al content. Consequently, the anatase-to-rutile transformation, generally observed for Ti1-xAlxN, is absent. This reduces the generation of pores and cracks within the oxide scale and especially at the nitride-oxide interface, leading to the formation of a protective rutile and corundum based oxide scale. This is also reflected in the pronounced decrease in activation energy for the protective scale formation from 232 kJ/mol for Ti0.35Al0.65N down to 14.5 kJ/mol for Ti0.32Al0.60Ta0.08N. Based on our results we can conclude that especially phase transformations within the oxide scale need to be suppressed, as the connected volume changes lead to the formation of cracks and pores.",1404.4345v1 2014-12-02,Effect of phase separation induced supercooling on magnetotransport properties of epitaxial La5/8-yPryCa3/8MnO3 (y~0.4) thin film,"Thin films of La5/8-yPryCa3/8MnO3 (y~0.4) have been grown on single crystal SrTiO3 (001) by RF sputtering. The structural and surface characterizations confirm the epitaxial nature of these film. However, the difference between the rocking curve of the (002) and (110) peaks and the presence of pits/holes in the step-terrace type surface morphology suggests high density of defect in these films. Pronounced hysteresis between the field cool cooled (FCC) and field cooled warming (FCW) magnetization measurements suggest towards the non-ergodic magnetic state. The origin of this nonergodicity could be traced to the magnetic liquid like state arising from the delicacy of the coexisting magnetic phases, viz., ferromagnetic and antiferromagnetic-charge ordered (FM/AFM-CO). The large difference between the insulator metal transitions during cooling and warming cycles (TIMC~64 K and TIMW~123 K) could be regarded as a manifestation of the nonergodicity leading to supercooling of the magnetic liquid while cooling. The nonergodicity and supercooling are weakened by the AFM-FM phase transition induced by an external magnetic field. TIM and small polaron activation energy corresponding the magnetic liquid state (cooling cycle) vary nonlinearly with the applied magnetic field but become linear in the crystalline solid state (warming cycle). The analysis of the low temperature resistivity data shows that electron-phonon interaction is drastically reduced by the applied magnetic field. The resistivity minimum in the lower temperature region of the self-field warming curve has been explained in terms of the Kondo like scattering in the magnetically inhomogeneous regime.",1412.0862v1 2016-11-09,Unusual non saturating Giant Magneto-resistance in single crystalline Bi2Te3 topological insulator,"We report synthesis, structural details and electrical transport properties of topological insulator Bi2Te3. The single crystalline specimens of Bi2Te3 are obtained from high temperature (950C) melt and slow cooling (2C/hour). The resultant crystals were shiny, one piece (few cm) and of bright silver color. The Bi2Te3 crystal is found to be perfect with clear [00l] alignment. The powder XRD pattern being carried out on crushed crystals showed that Bi2Te3 crystallized in R3m symmetry with a = b = 4.3866(2) A, c = 30.4978(13) A and Gamma = 120degree. The Bi position is refined to (0, 0, 0.4038 (9)) at Wyckoff position 6c and of Te are (0, 0, 0) at Wyckoff position 3a and at (0, 0, 0.2039(8)) at 6c. Ambient pressure and low temperature (down to 2K) electrical transport measurements revealed metallic behavior. Magneto transport measurements under magnetic field showed huge non saturating magneto resistance (MR) reaching up to 250% at 2.5K and under 50KOe field. Summarily, the short communication clearly demonstrates that Bi2Te3 topological insulator exhibit non-saturating large positive MR at low temperature of say below 10K. The non saturating MR is seen right up to room temperature albeit with much decreased magnitude. Worth mentioning is the fact that these crystals are bulk in nature and hence the anomalous MR is clearly an intrinsic property and not due to the size effect as reported for nano-wires or thin films of the same.",1611.02859v2 2016-11-28,Grand Design Spiral Arms in A Young Forming Circumstellar Disk,"We study formation and long-term evolution of a circumstellar disk in a collapsing molecular cloud core using a resistive magnetohydrodynamic simulation. While the formed circumstellar disk is initially small, it grows as accretion continues and its radius becomes as large as 200 AUs toward the end of the Class-I phase. A pair of grand-design spiral arms form due to gravitational instability in the disk, and they transfer angular momentum in the highly resistive disk. Although the spiral arms disappear in a few rotations as expected in a classical theory, new spiral arms form recurrently as the disk soon becomes unstable again by gas accretion. Such recurrent spiral arms persist throughout the Class-0 and I phase. We then perform synthetic observations and compare our model with a recent high-resolution observation of a young stellar object Elias 2-27, whose circumstellar disk has grand design spiral arms. We find good agreement between our theoretical model and the observation. Our model suggests that the grand design spiral arms around Elias 2-27 are consistent with material arms formed by gravitational instability. If such spiral arms commonly exist in young circumstellar disks, it implies that young circumstellar disks are considerably massive and gravitational instability is the key process of angular momentum transport.",1611.09361v2 2017-09-27,Pressure induced spin crossover in disordered α-LiFeO2,"Structural, magnetic and electrical-transport properties of {\alpha}-LiFeO2, crystallizing in the rock salt structure with random distribution of Li and Fe ions, have been studied by synchrotron X-ray diffraction, 57Fe M\""ossbauer spectroscopy and electrical resistance measurements at pressures up to 100 GPa using diamond anvil cells. It was found that the crystal structure is stable at least to 82 GPa, though a significant change in compressibility has been observed above 50 GPa. The changes in the structural properties are found to be on a par with a sluggish Fe3+ high- to low-spin (HS-LS) transition (S=5/2 to S=1/2) starting at 50 GPa and not completed even at ~100 GPa. The HS-LS transition is accompanied by an appreciable resistance decrease remaining a semiconductor up to 115 GPa and is not expected to be metallic even at about 200 GPa. The observed feature of the pressure-induced HS-LS transition is not an ordinary behavior of ferric oxides at high pressures. The effect of Fe3+ nearest and next nearest neighbors on the features of the spin crossover is discussed.",1709.09680v1 2018-03-24,Ion implantation in nanodiamonds: size effect and energy dependence,"Nanoparticles are ubiquitous in nature and are increasingly important for technology. They are subject to bombardment by ionizing radiation in a diverse range of environments. In particular, nanodiamonds represent a variety of nanoparticles of significant fundamental and applied interest. Here we present a combined experimental and computational study of the behaviour of nanodiamonds under irradiation by xenon ions. Unexpectedly, we observed a pronounced size effect on the radiation resistance of the nanodiamonds: particles larger than 8 nm behave similarly to macroscopic diamond (i.e. characterized by high radiation resistance) whereas smaller particles can be completely destroyed by a single impact from an ion in a defined energy range. This latter observation is explained by extreme heating of the nanodiamonds by the penetrating ion. The obtained results are not limited to nanodiamonds, making them of interest for several fields, putting constraints on processes for the controlled modification of nanodiamonds, on the survival of dust in astrophysical environments, and on the behaviour of actinides released from nuclear waste into the environment.",1803.09081v1 2020-09-14,Memristive control of mutual SHNO synchronization for neuromorphic computing,"Synchronization of large spin Hall nano-oscillators (SHNO) arrays is an appealing approach toward ultra-fast non-conventional computing based on nanoscale coupled oscillator networks. However, for large arrays, interfacing to the network, tuning its individual oscillators, their coupling, and providing built-in memory units for training purposes, remain substantial challenges. Here, we address all these challenges using memristive gating of W/CoFeB/MgO/AlOx based SHNOs. In its high resistance state (HRS), the memristor modulates the perpendicular magnetic anisotropy (PMA) at the CoFeB/MgO interface purely by the applied electric field. In its low resistance state (LRS), and depending on the voltage polarity, the memristor adds/subtracts current to/from the SHNO drive. The operation in both the HRS and LRS affects the SHNO auto-oscillation mode and frequency, which can be tuned up to 28 MHz/V. This tuning allows us to reversibly turn on/off mutual synchronization in chains of four SHNOs. We also demonstrate two individually controlled memristors to tailor both the coupling strength and the frequency of the synchronized state. Memristor gating is therefore an efficient approach to input, tune, and store the state of the SHNO array for any non-conventional computing paradigm, all in one platform.",2009.06594v1 2022-02-09,Electron-Electron Interaction and Weak Antilocalization Effect in a Transition Metal Dichalcogenide Superconductor,"In disordered transition-metal dichalcogenide (TMD) superconductor, both the strong spin-orbit coupling (SOC) and disorder show remarkable effects on superconductivity. However, the features of SOC and disorder were rarely detected directly. Here we report the quantum transport behaviors arising from the interplay of SOC and disorder in the TMD superconductor 1T-NbSeTe. Before entering the superconducting state, the single crystal at low temperature shows a resistivity upturn, which is T1/2 dependent and insensitive to the applied magnetic fields. The magnetoresistance (MR) at low temperatures shows a H1/2 dependence at high magnetic fields. The characteristics are in good agreement with the electron-electron interaction (EEI) in a disordered conductor. In addition, the upturn changes and MR at low magnetic fields suggest the contribution of weak antilocalization (WAL) effect arising from the strong SOC in the material. Moreover, the quantitative analyses of the transport features in different samples imply anomalous disorder-enhanced superconductivity that needs to be further understood. The results reveal the disorder enhanced EEI and the strong SOC induced WAL effect in 1T-NbSeTe, which illustrate the resistivity minimum in the widely studied doped superconductors. The work also provides insights into the disorder effect on the superconductivity.",2202.04338v1 2016-03-21,Measurement of Characteristic Impedance of Silicon Fiber Sheet based readout strips panel for RPC detector in INO,"The India based Neutrino Observatory (INO) is a mega science project of India, which is going to use near about 30, 000 Resistive Plate Chambers (RPC) as active detector elements for the study of atmospheric neutrino oscillations. Each RPC detector will consist of two orthogonally placed readout strips panel for picking the signals generated in the gas chamber. The area of RPC detector in INO-ICAL (Iron Calorimeter) experiment will be 2m x 2m, therefore the dimension of readout strips panel will also be of 2m x 2m. To get undistorted signals pass through the readout strips panel to frontend electronics, their Characteristic Impedance should be matched with each other. For the matching of Characteristic Impedance we have used the principle of termination. In the present paper we will describe the need and search of new dielectric material for the fabrication of flame resistant, waterproof and flexible readout pickup strips panel. We will also describe the measurement of Characteristic Impedance of plastic honeycomb based readout strips panel and Silicon Fiber sheet based readout strips panel in a comparative way, and its variation under loading and with time.",1603.06334v1 2017-04-18,Extruded Mg based hybrid composite alloys studied by longitudinal impression creep,"The creep behaviour of a creep-resistant AE42 magnesium alloy reinforced with Saffil short fibres and SiC particulates in various combinations has been examined in the longitudinal direction, i.e., the plane containing random fibre orientation was parallel to the loading direction, in the temperature range of 175-300 C at the stress levels ranging from 60 to 140 MPa using impression creep test technique. At 175 C, normal creep behaviour, i.e., strain rate decreasing with strain and then reaching a steady state, is observed at all the stresses employed. At 240 C, normal creep behaviour is observed up to 80 MPa and reverse creep behaviour, i.e., strain rate increasing with strain, then reaching a steady state and again decreasing, is observed above that stress. At 300 C, reverse creep behaviour is observed at all the stresses employed. This pattern remains the same for all the composites. The reverse creep behaviour is found to be associated with the fibre breakage. The stress exponent is found to be very high for all the composites. However, after taking the threshold stress into account, the stress exponent varies from 3.9 to 7.0, which suggests viscous glide and dislocation climb being the dominant creep mechanisms. The apparent activation energy Qc was not calculated due to insufficient data at any stress level either for normal or reverse creep behaviour. The creep resistance of the hybrid composites is found to be comparable to that of the composite reinforced with 20% Saffil short fibres at all the temperatures and stress levels investigated.",1704.06563v2 2018-08-12,High-pressure polymorphism of BaFe2Se3,"BaFe2Se3 is a potential superconductor material exhibiting transition at 11 K and ambient pressure. Here we extended the structural and performed electrical resistivity measurements on this compound up to 51 GPa and 20 GPa, respectively, in order to distinguish if the superconductivity in this sample is intrinsic to the BaFe2Se3 phase or if it is originating from minor FeSe impurities that show a similar superconductive transition temperature. The electrical resistance measurements as a function of pressure show that at 5 GPa the superconducting transition is observed at around 10 K, similar to the one previously observed for this sample at ambient pressure. This indicates that the superconductivity in this sample is intrinsic to the BaFe2Se3 phase and not to FeSe with Tc > 20 K at these pressures. Further increase in pressure suppressed the superconductive signal and the sample remained in an insulating state up to the maximum achieved pressure of 20 GPa. Single-crystal and powder X-ray diffraction measurements revealed two structural transformations in BaFe2Se3: a second order transition above 3.5 GPa from Pnma (CsAg2I3-type structure) to Cmcm (CsCu2Cl3-type structure) and a first order transformation at 16.6 GPa. Here, {\gamma}-BaFe2Se3 transforms into {\delta}-BaFe2Se3 (Cmcm, CsCu2Cl3-type average structure) via a first order phase transition mechanism. This transitions is characterized by a significant shortening of the b lattice parameter of {\gamma}-BaFe2Se3 (17%) and accompanied by an anisotropic expansion in the orthogonal ac plane at the transition point.",1808.03952v1 2019-03-14,Electric Switching of the Charge-Density-Wave and Normal Metallic Phases in Tantalum Disulfide Thin-Film Devices,"We report on switching among three charge-density-wave phases - commensurate, nearly commensurate, incommensurate - and the high-temperature normal metallic phase in thin-film 1T-TaS2 devices induced by application of an in-plane electric field. The electric switching among all phases has been achieved over a wide temperature range, from 77 K to 400 K. The low-frequency electronic noise spectroscopy has been used as an effective tool for monitoring the transitions, particularly the switching from the incommensurate charge-density-wave phase to the normal metal phase. The noise spectral density exhibits sharp increases at the phase transition points, which correspond to the step-like changes in resistivity. Assignment of the phases is consistent with low-field resistivity measurements over the temperature range from 77 K to 600 K. Analysis of the experimental data and calculations of heat dissipation suggest that Joule heating plays a dominant role in the electric-field induced transitions in the tested 1T-TaS2 devices on Si/SiO2 substrates. The possibility of electrical switching among four different phases of 1T-TaS2 is a promising step toward nanoscale device applications. The results also demonstrate the potential of noise spectroscopy for investigating and identifying phase transitions in materials.",1903.06050v1 2015-06-26,Negative Differential Resistance in Boron Nitride Graphene Heterostructures: Physical Mechanisms and Size Scaling Analysis,"Hexagonal boron nitride (hBN) is drawing increasing attention as an insulator and substrate material to develop next generation graphene-based electronic devices. In this paper, we investigate the quantum transport in heterostructures consisting of a few atomic layers thick hBN film sandwiched between graphene nanoribbon electrodes. We show a gate-controllable vertical transistor exhibiting strong negative differential resistance (NDR) effect with multiple resonant peaks, which stay pronounced for various device dimensions. We find two distinct mechanisms that are responsible for NDR, depending on the gate and applied biases, in the same device. The origin of first mechanism is a Fabry-P\'e like interference and that of the second mechanism is an in-plane wave vector matching when the Dirac points of the electrodes align. The hBN layers can induce an asymmetry in the current-voltage characteristics which can be further modulated by an applied bias. We find that the electron-phonon scattering introduces the decoherence and therefore suppresses first mechanism whereas second mechanism remains relatively unaffected. We also show that the NDR features are tunable by varying device dimensions. The NDR feature with multiple resonant peaks, combined with the ultrafast tunneling speed provides prospect for the graphene-hBN-graphene heterostructure in the high-performance electronics.",1506.08207v1 2015-07-02,Massive $2$-form field and holographic ferromagnetic phase transition,"In this paper, we investigate in some detail the holographic ferromagnetic phase transition in an AdS${_4}$ black brane background by introducing a massive 2-form field coupled to the Maxwell field strength in the bulk. In the two probe limits, one is to neglect the back reaction of the 2-form field to the background geometry and to the Maxwell field, and the other to neglect the back reaction of both the Maxwell field and the 2-form field, we find that the spontaneous magnetization and the ferromagnetic phase transition always happen when the temperature gets low enough with similar critical behavior. We calculate the DC resistivity in a semi-analytical method in the second probe limit and find it behaves as the colossal magnetic resistance effect in some materials. In the case with the first probe limit, we obtain the off-shell free energy of the holographic model near the critical temperature and compare with the Ising-like model. We also study the back reaction effect and find that the phase transition is always second order. In addition, we find an analytical Reissner-Norstr\""om-like black brane solution in the Einstein-Maxwell-2-form field theory with a negative cosmological constant.",1507.00546v2 2018-12-31,"Growth, Characterization and High Field Magneto-Conductivity of Co0.1Bi2Se3 Topological Insulator","We report the crystal growth as well as transport properties of Co added Bi2Se3 single crystals. The values of the lattice parameters a and b for Co added sample were observed to increase as compared to the pure Bi2Se3. The Raman spectroscopy displayed higher Raman shift of corresponding vibrational modes for Co0.1Bi2Se3, and the resistivity curves with and without applied magnetic field shows a metallic behaviour. Both the crystals were subjected to magneto-resistance (MR) measurements under applied fields of 14Tesla. The value of MR is found to decrease from about 380 (5K, 14 Tesla) for Bi2Se3 to 200 degree for Co0.1Bi2Se3. To elaborate the transport properties of pure and Co added Bi2Se3 crystals, the magneto-conductivity is fitted to the HLN (Hikami Larkin Nagaoka) equation and it is found that the charge conduction is mainly dominated by surface driven WAL (weak anti-localization) with negligible bulk WL (weak localization) contribution in both crystals alike. The MH curves of Co0.1Bi2Se3 crystal at different temperatures displayed a combination of both ferromagnetic and diamagnetic behaviour. On the other hand, the Electron Paramagnetic Resonance (EPR) revealed that pure Bi2Se3 is diamagnetic whereas, Co orders ferro-magnetically with resonating field around 3422Oe at room temperature.",1812.11713v1 2019-11-28,"Low-friction, wear-resistant, and electrically homogeneous multilayer graphene grown by chemical vapor deposition on molybdenum","Chemical vapour deposition (CVD) is a promising method for producing large-scale graphene (Gr). Nevertheless, microscopic inhomogeneity of Gr grown on traditional metal substrates such as copper or nickel results in a spatial variation of Gr properties due to long wrinkles formed when the metal substrate shrinks during the cooling part of the production cycle. Recently, molybdenum (Mo) has emerged as an alternative substrate for CVD growth of Gr, mainly due to a better matching of the thermal expansion coefficient of the substrate and Gr. We investigate the quality of multilayer Gr grown on Mo and the relation between Gr morphology and nanoscale mechanical and electrical properties, and spatial homogeneity of these parameters. With atomic force microscopy (AFM) based scratching, Kelvin probe force microscopy, and conductive AFM, we measure friction and wear, surface potential, and local conductivity, respectively. We find that Gr grown on Mo is free of large wrinkles that are common with growth on other metals, although it contains a dense network of small wrinkles. We demonstrate that as a result of this unique and favorable morphology, the Gr studied here has low friction, high wear resistance, and excellent homogeneity of electrical surface potential and conductivity.",1911.12653v1 2021-02-23,Strain-tuning of nematicity and superconductivity in single crystals of FeSe,"Strain is a powerful experimental tool to explore new electronic states and understand unconventional superconductivity. Here, we investigate the effect of uniaxial strain on the nematic and superconducting phase of single crystal FeSe using magnetotransport measurements. We find that the resistivity response to the strain is strongly temperature dependent and it correlates with the sign change in the Hall coefficient being driven by scattering, coupling with the lattice and multiband phenomena. Band structure calculations suggest that under strain the electron pockets develop a large in-plane anisotropy as compared with the hole pocket. Magnetotransport studies at low temperatures indicate that the mobility of the dominant carriers increases with tensile strain. Close to the critical temperature, all resistivity curves at constant strain cross in a single point, indicating a universal critical exponent linked to a strain-induced phase transition. Our results indicate that the superconducting state is enhanced under compressive strain and suppressed under tensile strain, in agreement with the trends observed in FeSe thin films and overdoped pnictides, whereas the nematic phase seems to be affected in the opposite way by the uniaxial strain. By comparing the enhanced superconductivity under strain of different systems, our results suggest that strain on its own cannot account for the enhanced high $T_c$ superconductivity of FeSe systems.",2102.11984v1 2021-02-24,Calibration of manganin pressure gauge for diamond-anvil cells,"Pressure calibration for most diamond-anvil cell (DAC) experiments is mainly based on the ruby scale, which is key to implement this powerful tool for high-pressure study. However, the ruby scale can often hardly be used for programmably-controlled DAC devices, especially the piezoelectric-driving cells, where a continuous pressure calibration is required. In this work, we present an effective pressure gauge for DACs made of manganin metal, based on the four-probe resistivity measurements. Pressure dependence of its resistivity is well established and shows excellent linear relations in the 0 - 30 GPa pressure range with a slope of 23.4 (9) GPa for the first-cycle compression, in contrast to that of multiple-cycle compression and decompression having a nearly identical slope of 33.7 (4) GPa likely due to the strain effect. In addition, such-established manganin scale can be used for continuously monitoring the cell pressure of piezoelectric-driving DACs, and the reliability of this method is also verified by the fixed-point method with a Bi pressure standard. Realization of continuous pressure calibration for programmably-controlled DACs would offer many opportunities for study of dynamics, kinetics, and critical behaviors of pressure-induced phase transitions.",2102.12125v1 2021-03-19,A Robust nitridation technique for fabrication of disordered superconducting TiN thin films featuring phase slip events,"Disorder induced phase slip (PS) events appearing in the current voltage characteristics (IVCs) are reported for two-dimensional TiN thin films produced by a robust substrate mediated nitridation technique. Here, high temperature annealing of Ti/Si3N4 based metal/substrate assembly is the key to produce majority phase TiN accompanied by TiSi2 and elemental Si as minority phases. The method itself introduces different level of disorder intrinsically by tuning the amount of the non-superconducting minority phases that are controlled by annealing temperature (Ta) and the film thickness. The superconducting critical temperature (Tc) strongly depends on Ta and the maximum Tc obtained from the demonstrated technique is about 4.8 K for the thickness range of about 12 nm and above. Besides, the dynamics of IVCs get modulated by the appearance of intermediated resistive steps for decreased Ta and the steps get more prominent for reduced thickness. Further, the deviation in the temperature dependent critical current (Ic) from the Ginzburg-Landau theoretical limit varies strongly with the thickness. Finally, the Tc, intermediate resistive steps in the IVCs and the depairing current are observed to alter in a similar fashion with Ta and the thickness indicating the robustness of the synthesis process to fabricate disordered nitride-based superconductor.",2103.10751v2 2021-07-22,Temperature dependence of on-state inter-terminal capacitances (Cgd and Cgs) of SiC MOSFETs and frequency limitations of their measurements,"Inter-terminal capacitances (ITCs) have major influence on the dynamic performance of power SiC MOSFETs. Knowledge of the exact values for the ITCs is required in order to perform accurate and predictive compact model simulations of their dynamic performance. Since commercial SiC MOSFETs are capable of operating in a wide range of temperatures, it is important to know the values of ITCs in the whole temperature range of operation. Direct measurements of the ITCs with standard equipment is possible only at low current levels (i.e. in the off-state (Vgs < Vth) for Vds > 0 V), however their values in the on-state (Vgs>Vth) also influence the MOSFETs switching performance. In this work, ITCs of a planar SiC MOSFET in the on-state are studied by the means of a calibrated TCAD model, revealing substantial temperature dependence in the range of 300-450 K. In the first approximation, this temperature dependence of the ITCs can be explained by a weaker temperature dependence of the MOSFET channel resistance in comparison to its JFET and epitaxial layer resistances. In addition, it is shown that at high frequencies stray inductances of the TO-247-3 package result in a change of the extracted values of the on-state ITCs. This effect is already notable at 1 MHz.",2107.10408v1 2021-07-24,Anomalous Nernst thermopower and giant magnetostriction in microwave synthesized La0.5Sr0.5CoO3,"Ferromagnetic metallic oxides have potential applications in spincaloric devices which utilize the spin property of charge carriers for interconversion of heat and electricity through the spin Seebeck or the anomalous Nernst effect or both. In this work, we synthesized polycrystalline La0.5S0.5CoO3 by microwave irradiation method and studied its transverse thermoelectric voltage (Nernst thermopower) and change in the linear dimension of the sample (Joule magnetostriction) in response to external magnetic fields. In addition, magnetization, temperature dependences of electrical resistivity, and longitudinal Seebeck coefficient (Sxx) in absence of an external magnetic field were also measured. The sample is ferromagnetic with a Curie temperature of TC = 247 K and shows a metal-like resistivity above and below TC with a negative sign of Sxx suggesting charge transport due to electrons. Magnetic field dependence of the Nernst thermopower (Sxy) at a fixed temperature shows a rapid increase at low fields and a tendency to saturate at high fields as like the magnetization. Anomalous contribution to Sxy was extracted from total Sxy measured and it exhibits a maximum value of ~ 0.21 microV/K at 180 K for H = 50 kOe, which is comparable to the value found in a single crystal for a lower Sr content. The Joule magnetostriction is positive, i.e., the length of the sample expands along the direction of the magnetic field and it does not saturate even at 50 kOe. The magnetostriction increases with decreasing temperature below TC and reaches a maximum value of 500 ppm at T = 40 K and below. Coexistence of the anomalous Nernst thermopower and giant magnetostriction in a single compound has potential applications for thermal energy harvesting and low-temperature actuators, respectively.",2107.11535v1 2022-01-15,Fabrication and micro-Raman spectroscopy of arrays of copper phthalocyanine molecular-magnet microdisks,"Phthalocyanines as organic semiconductors and molecular magnets provide plenty of industrial or high-tech applications from dyes and pigments up to gas sensors, molecular electronics, spintronics and quantum computing. Copper phthalocyanine (CuPc) belongs among the most used phthalocyanines, typically in the form of powder or films but self-grown nanowires are also known. Here we describe an opposite, i.e., top-down approach based on fabrication of ordered arrays of CuPc microstructures (microdisks) using electron beam lithography and other steps. Among critical points of this approach belongs a choice of a proper resist and a solvent. Fabricated CuPc microdisks have a diameter of 5 ${\mu}$m and heights from 7 up to 70 nm. Micro-Raman spectroscopy of the films and microdisks reveals a crystalline ${\beta}$ phase associated with a paramagnetic form. Additional measurements with an increasing laser power show a significant shift (${\Delta}{\omega}$ ~ 7.1 cm$^{-1}$ ) and broadening of a peak at 1532 rel$\cdot$cm$^{-1}$ corresponding to the phonon B1g mode. The observed smooth changes exclude a phase transition and confirm the thermally stable polymorph. Our versatile fabrication technique using the common lithographic resist brings new possibilities for the fabrication of various micro/nanostructures such as micromagnets, heterostructures or organic electronic devices.",2201.08235v1 2022-07-06,Mechanism of the Resistivity Switching Induced by the Joule Heating in Crystalline NbO$_2$,"Recently the memristive electrical transport properties in NbO$_2$ have attracted much attention for their promising application to the neuromorphic computation. At the center of debates is whether the metal-to-insulator transition (MIT) originates from the structural distortion (Peierls) or the electron correlation (Mott). With inputs from experiments and first principles calculations, we develop a thermodynamical model rooted in the scenario of the MIT driven by a $2^{nd}$ order Peierls instability. We find that the temperature dependence of the electrical conductivity can be accurately fit by the band gap varying with temperature due to the gradual weakening of the Nb-Nb dimers. The resistivity switching can consequently be understood by dimer-free metallic domains induced by local Joule heating. In solving the heat equation, we find that the steady state can not be reached if the applied voltage exceeds a threshold, resulting in the chaotic behavior observed in the high voltage and current states. With the Ginzburg-Landau theory and the Joule heating equation, the evolution of the metallic domains under bias voltage can be simulated and directly verified by experiments.",2207.02682v2 2022-12-13,Deep multilevel wet etching of fused silica glass microstructures in BOE solution,"Fused silica glass is a material of choice for micromechanical, microfluidic, and optical devices due to its ultimate chemical resistance, optical, electrical, and mechanical performance. Wet etching in hydrofluoric solutions especially a buffered oxide etching (BOE) solution is still the key method for fabricating fused silica glass-based microdevices. It is well known that protective mask integrity during deep fused silica wet etching is a big challenge due to chemical stability of fused glass and extremely aggressive BOE properties. Here, we propose a multilevel fused silica glass microstructures fabrication route based on deep wet etching through a stepped mask with just a one grayscale photolithography step. First, we provide a deep comprehensive analysis of a fused quartz dissolution mechanism in BOE solution and calculate the main fluoride fractions like $HF^-_2$, $F^-$, $(HF)_2$ components in a BOE solution as a function of pH and $NH_4F:HF$ ratio at room temperature. Then, we experimentally investigate the influence of BOE concentration ($NH_4F:HF$ from 1:1 to 14:1) on the mask resistance, etch rate and profile isotropy during fused silica 60 minutes etching through a metal/photoresist mask. Finally, we demonstrate a high-quality multilevel over-200 um isotropic wet etching process with the rate up to 3 um/min, which could be of a great interest for advanced fused silica microdevices with flexure suspensions, inertial masses, microchannels, and through-wafer holes.",2212.06699v1 2023-03-02,Evolution of complex magnetic phases and metal-insulator transition through Nb substitution in La$_{0.5}$Sr$_{0.5}$Co$_{1-x}$Nb$_x$O$_3$,"We report the evolution of structural, magnetic, transport, and electronic properties of bulk polycrystalline La$_{0.5}$Sr$_{0.5}$Co$_{1-x}$Nb$_x$O$_3$ ($x =$ 0.025--0.25) samples. The Rietveld refinement of the x-ray diffraction patterns with R$\bar3$c space group reveals that the lattice parameters and rhombohedral distortion monotonously increase with the Nb$^{5+}$(4$d^0$) substitution ($x$). The magnetic susceptibility exhibits a decrease in the magnetic ordering temperature and net magnetization with $x$, which manifests that the Nb substitution dilutes the ferromagnetic (FM) double exchange interaction and enhances the antiferromagnetic (AFM) super-exchange interaction. Interestingly, for the $x>$ 0.1 samples the FM order is completely suppressed and the emergence of a glassy state is clearly evident. Moreover, the decrease in the coercivity (H$\rm_{C}$) and remanence (M$\rm_{r}$) with $x$ in the magnetic isotherms measured at 5~K further confirms the dominance of AFM interactions and reduction of FM volume fraction for the $x>$ 0.1 samples. More interestingly, we observe resistivity minima for the $x=$ 0.025 and 0.05 samples, which are analyzed using the quantum corrections in the conductivity, and found that the weak localization effect dominates over the renormalized electron-electron interactions in the 3D limit. Further, a semiconducting resistivity behavior is obtained for $x>$ 0.05, which follows the Arrhenius law at high temperatures ($\sim$160--320~K), and the 3D-variable range hopping prevails in the low-temperature region ($<$160~K). The core-level photoemission spectra confirm the valence state of constituent elements and the absence of Co$^{2+}$ is discernible.",2303.01108v1 2023-10-18,Electrically-driven amplification of terahertz acoustic waves in graphene,"In graphene devices, the electronic drift velocity can easily exceed the speed of sound in the material at moderate current biases. Under this condition, the electronic system can efficiently amplify acoustic phonons, leading to the exponential growth of sound waves in the direction of the carrier flow. Here, we demonstrate that such phonon amplification can significantly modify the electrical properties of graphene devices. We observe a super-linear growth of the resistivity in the direction of the carrier flow when the drift velocity exceeds the speed of sound, causing up to a 7 times increase over 8 micrometers. The resistance growth is observable for carrier densities away from the Dirac point and is enhanced at cryogenic temperatures. These observations are explained by a theoretical model for the electrical-amplification of acoustic phonons, which reach frequencies up to 2.2 terahertz with the nanoscale wavelength set by gate-tunable ~kF transitions across the Fermi surface. These findings offer a route to high-frequency on-chip sound generation and detection, which can be used to modulate and probe electronic physics in van der Waals heterostructures in the terahertz frequency range.",2310.12225v1 2024-04-24,Structural investigation of the quasi-one-dimensional topological insulator Bi$_4$I$_4$,"The bismuth-halide Bi$_4$I$_4$ undergoes a structural transition around $T_P\sim 300$K, which separates a high-temperature $\beta$ phase ($T>T_P$) from a low-temperature $\alpha$ phase ($T 0.01. Such a very weak solubility limit could also be responsible for the discrepancies found in the literature. Furthermore, the measurements made under magnetic field (magnetic susceptibility, electrical resistivity and Seebeck coefficient) support that the Cr^4+ ""holes"", created by the Mg^2+ substitution, in the matrix of high spin Cr^3+ (S = 3/2) are responsible for the transport properties of these compounds.",0908.3828v1 2009-12-02,Magnetotransport of La0.70ca0.3-xsrxmno3 (Ag): A Potential Room Temperature Bolometer and Magnetic Sensor,"Here we report the optimized magneto-transport properties of polycrystalline La0.70Ca0.3-xSrxMnO3 and their composites with Ag. The optimization was carried out by varying the Sr and Ag contents simultaneously to achieve large temperature coefficient of resistance (TCR) as well as low field magneto-resistance (MR) at room temperature. Sharpest paramagnetic (PM)-ferromagnetic (FM) and insulator-metal (IM) transition is observed in the vicinity of the room temperature (TC=300 K=TIM) for the composition La0.70Ca0.20Sr00.10MnO3:Ag0.20. Partial substitution of larger Sr2+ ions at the Ca2+ ions sites controls the magnitude of the FM and IM transition temperatures, while the Ag induces the desired sharpness in these transitions. For the optimized composition, maximum TCR and MR are tuned to room temperature (300 K) with the former being as high as 9% and the later being 20 and 30 percent at 5 and 10 kOe magnetic fields respectively. Such sharp single peak (TCR= 9 percent) at room temperature can be used for the bolometric and infrared detector applications. The achievement of large TCR and low field MR at T~300K in polycrystalline samples is encouraging and we believe that further improvements can be achieved in thin films, which, by virtue of their low conduction noise, are more suitable for device applications.",0912.0347v2 2012-08-16,Gate tunable quantum transport in double layer graphene,"We analyze the effect of screening provided by the additional graphene layer in double layer graphene heterostructures (DLGs) on transport characteristics of DLG devices in the metallic regime. The effect of gate-tunable charge density in the additional layer is two-fold: it provides screening of the long-range potential of charged defects in the system, and screens out Coulomb interactions between charge carriers. We find that the efficiency of defect charge screening is strongly dependent on the concentration and location of defects within the DLG. In particular, only a moderate suppression of electron-hole puddles around the Dirac point induced by the high concentration of remote impurities in the silicon oxide substrate could be achieved. A stronger effect is found on the elastic relaxation rate due to charged defects resulting in mobility strongly dependent on the electron denisty in the additional layer of DLG. We find that the quantum interference correction to the resistivity of graphene is also strongly affected by screening in DLG. In particular, the dephasing rate is strongly suppressed by the additional screening that supresses the amplitude of electron-electron interaction and reduces the diffusion time that electrons spend in proximity of each other. The latter effect combined with screening of elastic relaxation rates results in a peculiar gate tunable weak-localization magnetoresistance and quantum correction to resistivity. We propose suitable experiments to test our theory and discuss the possible relevance of our results to exisiting data.",1208.3470v2 2012-10-20,Tunable spin reorientation transition and magnetocaloric effect in Sm0.7-xLaxSr0.3MnO3 series,"We report electrical resistivity, magnetic and magnetocaloric properties in Sm0.7-xLaxSr0.3MnO3 series for x= 0, 0.1, 0.2, 0.3, 0.4, 0.5, 0.6, 0.65, and 0.7. All the compounds show second order paramagnetic to ferromagnetic transition at T = Tc which is tunable anywhere between 83 K and 373 K with a proper choice of the doping level (x). The insulating ferromagnet x= 0 transforms to ferromagnetic metal below Tc for x= 0.1 and the insulator-metal transition temperature shifts up with increasing x. The magnetization (M) exhibits an interesting behavior as a function of temperature and doping level. The field-cooled M(T) of all but x= 0.7 compound show a cusp at a temperature T* much below Tc. While the Tc increases monotonically with increasing x, T* increases gradually, attains a maximum value (T*= 137 K) for x= 0.6 and decreases rapidly thereafter. It is suggested that the decrease of M(T) below T* is due to ferrimagnetic interaction between Sm(4f) and Mn(3d) sublattices that promotes spin-reorientation transition of the Mn-sublattice. The observed anomalous feature in M(T) does not have impact on the dc resistivity. Magnetic entropy change (delta Sm) was estimated from magnetization isotherms. The sign of delta Sm is found to change from negative above T* to positive below T* indicating the coexistence of normal and inverse magnetocaloric effects. delta Sm is nearly composition independent (-delta Sm is about 1.5 J/Kg K for delta H = 1 Tesla) and refrigeration capacity lies between 50 and 80 J/kg K for x = 0.1-0.6. The tunability of Curie temperature with a nearly constant delta Sm value along with high refrigeration capacity makes this series of compounds interesting for magnetic refrigeration over a wide temperature range.",1210.5595v1 2012-11-27,"Anisotropic Impurity-States, Quasiparticle Scattering and Nematic Transport in Underdoped Ca(Fe1-xCox)2As2","Iron-based high temperature superconductivity develops when the `parent' antiferromagnetic/orthorhombic phase is suppressed, typically by introduction of dopant atoms. But their impact on atomic-scale electronic structure, while in theory quite complex, is unknown experimentally. What is known is that a strong transport anisotropy with its resistivity maximum along the crystal b-axis, develops with increasing concentration of dopant atoms; this `nematicity' vanishes when the `parent' phase disappears near the maximum superconducting Tc. The interplay between the electronic structure surrounding each dopant atom, quasiparticle scattering therefrom, and the transport nematicity has therefore become a pivotal focus of research into these materials. Here, by directly visualizing the atomic-scale electronic structure, we show that substituting Co for Fe atoms in underdoped Ca(Fe1-xCox)2As2 generates a dense population of identical anisotropic impurity states. Each is ~8 Fe-Fe unit cells in length, and all are distributed randomly but aligned with the antiferromagnetic a-axis. By imaging their surrounding interference patterns, we further demonstrate that these impurity states scatter quasiparticles in a highly anisotropic manner, with the maximum scattering rate concentrated along the b-axis. These data provide direct support for the recent proposals that it is primarily anisotropic scattering by dopant-induced impurity states that generates the transport nematicity; they also yield simple explanations for the enhancement of the nematicity proportional to the dopant density and for the occurrence of the highest resistivity along the b-axis.",1211.6454v1 2013-05-16,Different routes to pressure-induced volume collapse transitions in gadolinium and terbium metals,"The sudden decrease in molar volume exhibited by most lanthanides under high pressure is often attributed to changes in the degree of localization of their 4f-electrons. We give evidence, based on electrical resistivity measurements of dilute Y(Gd) and Y(Tb) alloys to 120 GPa, that the volume collapse transitions in Gd and Tb metals have different origins, despite their being neighbors in the periodic table. Remarkably, the change under pressure in the magnetic state of isolated Pr or Tb impurity ions in the nonmagnetic Y host appears to closely mirror corresponding changes in pure Pr or Tb metals. The collapse in Tb appears to be driven by an enhanced negative exchange interaction between 4f and conduction electrons under pressure (Kondo resonance) which, in the case of Y(Tb), dramatically alters the superconducting properties of the Y host, much like previously found for Y(Pr). In Gd our resistivity measurements suggest that a Kondo resonance is not the main driver for its volume collapse. X-ray absorption and emission spectroscopies clearly show that 4f local moments remain largely intact across both volume collapse transitions ruling out 4f band formation (delocalization) and valence transition models as possible drivers. The results highlight the richness of behavior behind the volume collapse transition in lanthanides and demonstrate the stability of the 4f level against band formation to extreme pressure.",1305.3852v4 2014-04-09,Quantum transport evidence for a three-dimensional Dirac semimetal phase in Cd3As2,"The material termed three-dimensional (3D) Dirac semimetal has attracted great interests recently, since it is an electronic analogue to two-dimensional graphene. Starting from this novel phase, various topologically distinct phases may be obtained, such as topological insulator, Weyl semimetal, quantum spin Hall insulator, and topological superconductor. Soon after the theoretical predictions, the angle-resolve photoemission spectroscopy and scanning tunnelling microscopy experiments gave evidences for 3D Dirac points in Na3Bi and Cd3As2. Here we report quantum transport properties of Cd3As2 single crystal in magnetic field. A sizable linear quantum magnetoresistance is observed at high temperature. With decreasing temperature, the Shubnikov-de Haas oscillations appear in both longitudinal resistance Rxx and transverse Hall resistance Rxy. From the strong oscillatory component \Delta Rxx, the linear dependence of Landau index n on 1/B gives an n-axis intercept 0.58. Our quantum transport result clearly reveals a nontrivial \pi\ Berry's phase, thus provides strong bulk evidence for a 3D Dirac semimetal phase in Cd3As2. This may open new perspectives for its use in electronic devices.",1404.2557v3 2014-04-15,Formation of a topological non-Fermi liquid in MnSi,"Fermi liquid theory provides a remarkably powerful framework for the description of the conduction electrons in metals and their ordering phenomena, such as superconductivity, ferromagnetism, and spin- and charge-density-wave order. A different class of ordering phenomena of great interest concerns spin configurations that are topologically protected, that is, their topology can be destroyed only by forcing the average magnetization locally to zero. Examples of such configurations are hedgehogs (points at which all spins are either pointing inwards or outwards) or vortices. A central question concerns the nature of the metallic state in the presence of such topologically distinct spin textures. Here we report a high-pressure study of the metallic state at the border of the skyrmion lattice in MnSi, which represents a new form of magnetic order composed of topologically non-trivial vortices. When long-range magnetic order is suppressed under pressure, the key characteristic of the skyrmion lattice - that is, the topological Hall signal due to the emergent magnetic flux associated with their topological winding - is unaffected in sign or magnitude and becomes an important characteristic of the metallic state. The regime of the topological Hall signal in temperature, pressure and magnetic field coincides thereby with the exceptionally extended regime of a pronounced non-Fermi-liquid resistivity. The observation of this topological Hall signal in the regime of the NFL resistivity suggests empirically that spin correlations with non-trivial topological character may drive a breakdown of Fermi liquid theory in pure metals.",1404.4050v1 2014-09-12,Observation of topological surface state quantum Hall effect in an intrinsic three-dimensional topological insulator,"A three-dimensional (3D) topological insulator (TI) is a quantum state of matter with a gapped insulating bulk yet a conducting surface hosting topologically-protected gapless surface states. One of the most distinct electronic transport signatures predicted for such topological surface states (TSS) is a well-defined half-integer quantum Hall effect (QHE) in a magnetic field, where the surface Hall conductivities become quantized in units of (1/2)e2/h (e being the electron charge, h the Planck constant) concomitant with vanishing resistance. Here, we observe well-developed QHE arising from TSS in an intrinsic TI of BiSbTeSe2. Our samples exhibit surface dominated conduction even close to room temperature, while the bulk conduction is negligible. At low temperatures and high magnetic fields perpendicular to the top and bottom surfaces, we observe well-developed integer quantized Hall plateaus, where the two parallel surfaces each contributing a half integer e2/h quantized Hall (QH) conductance, accompanied by vanishing longitudinal resistance. When the bottom surface is gated to match the top surface in carrier density, only odd integer QH plateaus are observed, representing a half-integer QHE of two degenerate Dirac gases. This system provides an excellent platform to pursue a plethora of exotic physics and novel device applications predicted for TIs, ranging from magnetic monopoles and Majorana particles to dissipationless electronics and fault-tolerant quantum computers.",1409.3778v2 2014-12-23,Magnetic and structural transitions in La$_{0.4}$Na$_{0.6}$Fe$_2$As$_2$ single crystals,"La$_{0.4}$Na$_{0.6}$Fe$_2$As$_2$ single crystals have been grown out of an NaAs flux in an alumina crucible and characterized by measuring magnetic susceptibility, electrical resistivity, specific heat, as well as single crystal x-ray and neutron diffraction. La$_{0.4}$Na$_{0.6}$Fe$_2$As$_2$ single crystals show a structural phase transition from a high temperature tetragonal phase to a low-temperature orthorhombic phase at T$_s$\,=\,125\,K. This structural transition is accompanied by an anomaly in the temperature dependence of electrical resistivity, anisotropic magnetic susceptibility, and specific heat. Concomitant with the structural phase transition, the Fe moments order along the \emph{a} direction with an ordered moment of 0.7(1)\,$\mu_{\textup{B}}$ at \emph{T}\,=\,5 K. The low temperature stripe antiferromagnetic structure is the same as that in other \emph{A}Fe$_{2}$As$_{2}$ (\emph{A}\,=\,Ca, Sr, Ba) compounds. La$_{0.5-x}$Na$_{0.5+x}$Fe$_2$As$_2$ provides a new material platform for the study of iron-based superconductors where the electron-hole asymmetry could be studied by simply varying La/Na ratio.",1412.7447v1 2015-01-08,Structure and bonding in amorphous iron carbide thin films,"We investigate the amorphous structure, chemical bonding, and electrical properties of magnetron sputtered Fe1-xCx (0.21120K, the opposite temperature dependence of resistance for in up and down ferroelectric polarization states results in a rapid diminishing of tunneling electroresistance (TER). These results contribute to the understanding of the transport properties for designing high performance OMFTJs for memristor and spintronics applications.",2004.03284v1 2020-09-16,"High Field Magneto-Transport of Mixed Topological Insulators Bi2Se3-xTex (x = 0, 1, 2 & 3)","The article comprises structural, microstructural, and physical properties analysis of Bi2Se3-xTex (x= 0, 1, 2 and 3) mixed topological insulator (MTI) single crystals. All the crystals were grown through a well-optimized solid-state reaction route via the self-flux method. These MTI are well characterized through XRD (X-ray Diffraction), SEM (Scanning Electron Microscopy), EDAX (Energy Dispersive spectroscopy), and thereby, the physical properties are analyzed through the RT (Resistance vs temperature) down to 10K as well as the magneto-resistance (MR) measurements (at 5K) in a magnetic field of up to 10 Tesla. The MR drastically varies from x=0 to x=3 in MTI, from a huge 400 percent, it goes down to 20 percent and 5 percent and eventually back to 315 percent. This fascinated behaviour of MR is explained in this article through HLN (Hikami-Larkin-Nagaoka) equation and an additional term. This article not only proposed the mesmerizing behavior of MR in MTI but also explains the reason through competing WAL (Weak Anti-Localization) and WL (Weak Localization) conduction processes.",2009.07757v1 2016-03-05,Development and characterization of single gap glass RPC,"India-based Neutrino Observatory (INO) facility is going to have a 50 kton magnetized Iron CALorimeter (ICAL) detector for precision measurements of neutrino oscillations using atmospheric neutrinos. The proposed ICAL detector will be a stack of magnetized iron plates (acting as target material) interleaved with glass Resistive Plate Chambers (RPCs) as the active detector elements. An RPC is a gaseous detector made up of two parallel electrode plates having high bulk resistivity like that of float glass and bakelite. For the ICAL detector, glass is preferred over bakelite as it does not need any kind of surface treatment to achieve better surface uniformity and also the cost of associated electronics is reduced. Under the detector R&D efforts for the proposed glass RPC detector, a few glass RPCs of 1m X 1m dimension are fabricated procuring glass of ~ 2 mm thickness from one of the Indian glass manufacturers (Asahi). In the present paper, we report the characterization of RPC based on leakage current study, muon detection efficiency and noise rate studies with varying gas compositions.",1603.01719v5 2017-08-08,High Surface Conductivity of Fermi Arc Electrons in Weyl semimetals,"Weyl semimetals (WSMs), a new type of topological condensed matter, are currently attracting great interest due to their unusual electronic states and intriguing transport properties such as chiral anomaly induced negative magnetoresistance, a semi--quantized anomalous Hall effect and the debated chiral magnetic effect. These systems are close cousins of topological insulators (TIs) which are known for their disorder tolerant surface states. Similarly, WSMs exhibit unique topologically protected Fermi arcs surface states. Here we analyze electron--phonon scattering, a primary source of resistivity in metals at finite temperatures, as a function of the shape of the Fermi arc where we find that the impact on surface transport is significantly dependent on the arc curvature and disappears in the limit of a straight arc. Next, we discuss the effect of strong surface disorder on the resistivity by numerically simulating a tight binding model with the presence of quenched surface vacancies using the Coherent Potential Approximation (CPA) and Kubo--Greenwood formalism. We find that the limit of a straight arc geometry is remarkably disorder tolerant, producing surface conductivity that is a factor of 50 larger of a comparable set up with surface states of TI. Finally, a simulation of the effects of surface vacancies on TaAs is presented, illustrating the disorder tolerance of the topological surface states in a recently discovered WSM material.",1708.02415v1 2019-08-21,Half-metallic ferromagnetism and Ru-induced localization in quaternary Heusler alloy CoRuMnSi,"We report a combined theoretical and experimental investigation of half-metallic ferromagnetism in equiatomic quaternary Heusler alloy CoRuMnSi. Room temperature XRD analysis reveals that the alloy crystallizes in L21 disorder instead of pristine Y-type structure due to 50% swap disorder between the tetrahedral sites, i.e., Co and Ru atoms. Magnetization measurements reveal a net magnetization of 4 $\mu_B$ with Curie temperature of ~780 K. Resistivity measurement reveals the presence of localization effect below 35 K while above 100 K, a linear dependence is observed. Resistivity behavior indicates the absence of single magnon scattering, which indirectly supports the half-metallic nature. The majority spin band near the Fermi level clearly indicates the overlap of flat eg bands with sharply varying conduction bands that are responsible for the localization. In-depth analysis of the projected atomic d-orbital character of band structure reveals unusual bonding, giving rise to the flat eg bands purely arising out of Ru ions. Co-Ru swap disorder calculations indicate the robustness of half-metallic nature, even when the structure changes from Y-type to L21-type, with no major change in the net magnetization of the system. Thus, robust half-metallic nature, stable structure, and high Curie temperature make this alloy quite a promising candidate to be used as a source of highly spin-polarized currents in spintronic applications.",1908.07804v1 2012-03-10,How local is the Phantom Force?,"The phantom force is an apparently repulsive force, which can dominate the atomic contrast of an AFM image when a tunneling current is present. We described this effect with a simple resistive model, in which the tunneling current causes a voltage drop at the sample area underneath the probe tip. Because tunneling is a highly local process, the areal current density is quite high, which leads to an appreciable local voltage drop that in turn changes the electrostatic attraction between tip and sample. However, Si(111)-7\times7 has a metallic surface-state and it might be proposed that electrons should instead propagate along the surface-state, as through a thin metal film on a semiconducting surface, before propagating into the bulk. In this article, we investigate the role of the metallic surface-state on the phantom force. First, we show that the phantom force can be observed on H/Si(100), a surface without a metallic surface-state. Furthermore, we investigate the influence of the surface-state on our phantom force observations of Si(111)-7\times7 by analyzing the influence of the macroscopic tip radius R on the strength of the phantom force, where a noticeable effect would be expected if the local voltage drop would reach extensions comparable to the tip radius. We conclude that a metallic surface-state does not suppress the phantom force, but that the local resistance Rs has a strong effect on the magnitude of the phantom force.",1203.2258v1 2012-06-14,Influence of the substrate and precursor on the magnetic and magneto-transport properties in magnetite films,"We have investigated the magnetic and transport properties of nanoscaled Fe3O4 films obtained from Chemical Vapor Deposition (CVD) technique using [FeIIFe2III(OBut)8] and [Fe2III(OBut)6] precursors. Samples were deposited on different substrates (i.e., MgO (001), MgAl2O4 (001) and Al2O3 (0001)) with thicknesses varying from 50 to 350 nm. Atomic Force Microscopy analysis indicated a granular nature of the samples, irrespective of the synthesis conditions (precursor and deposition temperature, Tpre) and substrate. Despite the similar morphology of the films, magnetic and transport properties were found to depend on the precursor used for deposition. Using [FeIIFe2III(OBut)8] as precursor resulted in lower resistivity, higher MS and a sharper magnetization decrease at the Verwey transition (TV). The temperature dependence of resistivity was found to depend on the precursor and Tpre. We found that the transport is dominated by the density of antiferromagnetic antiphase boundaries (AF-APB's) when [FeIIFe2III(OBut)8] precursor and Tpre = 363 K are used. On the other hand, grain boundary-scattering seems to be the main mechanism when [Fe2III(OBut)6] is used. The Magnetoresistance (MR(H)) displayed an approximate linear behavior in the high field regime (H > 796 kA/m), with a maximum value at room-temperature of \sim2-3% for H = 1592 kA/m, irrespective from the transport mechanism.",1206.3158v1 2015-07-23,Percolative Metal-Insulator Transition in LaMnO$_3$,"We show that the pressure-induced metal-insulator transition (MIT) in LaMnO$_3$ is fundamentally different from the Mott-Hubbard transition and is percolative in nature, with the measured resistivity obeying the percolation scaling laws. Using the Gutzwiller method to treat correlation effects in a model Hamiltonian that includes both Coulomb and Jahn-Teller interactions, we show, One, that the MIT is driven by a competition between electronic correlation and the electron-lattice interaction, an issue that has been long debated, and Two, that with compressed volume, the system has a tendency towards phase separation into insulating and metallic regions, consisting, respectively, of Jahn-Teller distorted and undistorted octahedra. This tendency manifests itself in a mixed phase of intermixed insulating and metallic regions in the experiment. Conduction in the mixed phase occurs by percolation and the MIT occurs when the metallic volume fraction, steadily increasing with pressure, exceeds the percolation threshold $v_c \approx 0.29$. Measured high-pressure resistivity follows the percolation scaling laws quite well, establishing the percolative nature of conduction, and the temperature dependence follows the Efros-Shklovskii variable-range hopping behavior for granular materials.",1507.06592v2 2019-06-20,On the interaction of precipitates and tensile twins in magnesium alloys,"Although magnesium alloys deform extensively through shear strains and crystallographic re-orientations associated with the growth of twins, little is known about the strengthening mechanisms associated with this deformation mode. A crystal plasticity based phase field model for twinning is employed in this work to study the strengthening mechanisms resulting from the interaction between twin growth and precipitates. The full-field simulations reveal in great detail the pinning and de-pinning of a twin boundary at individual precipitates, resulting in a maximum resistance to twin growth when the precipitate is partially embedded in the twin. Furthermore, statistically representative precipitate distributions are used to systematically investigate the influence of key microstructural parameters such as precipitate orientation, volume fraction, size, and aspect ratio on the resistance to twin growth. The results indicate that the effective critical resolved shear stress (CRSS) for twin growth increases linearly with precipitate volume fraction and aspect ratio. For a constant volume fraction of precipitates, reduction of the precipitate size below a critical level produces a strong increase in the CRSS due to the Orowan-like strengthening mechanism between the twin interface and precipitates. Above this level the CRSS is size independent. The results are quantitatively and qualitatively comparable with experimental measurements and predictions of mean-field strengthening models. Based on the results, guidelines for the design of high strength magnesium alloys are discussed.",1906.08736v2 2020-01-15,Ohmic contacts on n-type and p-type cubic silicon carbide (3C-SiC) grown on silicon,"This paper is a report on Ohmic contacts on n-type and p-type type cubic silicon carbide (3C-SiC) layers grown on silicon substrates. In particular, the morphological, electrical and structural properties of annealed Ni and Ti/Al/Ni contacts has been studied employing several characterization techniques. Ni films annealed at 950{\deg}C form Ohmic contacts on moderately n-type doped 3C-SiC (ND ~ 1x1017cm-3), with a specific contact resistance of 3.7x10-3 {\Omega}cm2. The main phase formed upon annealing in this contact was nickel silicide (Ni2Si), with randomly dispersed carbon in the reacted layer. In the case of a p-type 3C-SiC with a high doping level (NA ~ 5x1019cm-3), Ti/Al/Ni contacts were preferable to Ni ones, as they gave much lower values of the specific contact resistance (1.8x10-5 {\Omega}cm2). Here, an Al3Ni2 layer was formed in the uppermost part of the contact, while TiC was detected at the interface. For this system, a temperature dependent electrical characterization allowed to establish that the thermionic field emission rules the current transport at the interface. All these results can be useful for the further development of a devices technology based on the 3C-SiC polytype.",2001.05159v4 2020-01-22,Correlation between crystal purity and the charge density wave in 1$T$-VSe$_2$,"We examine the charge density wave (CDW) properties of 1$T$-VSe$_{2}$ crystals grown by chemical vapour transport (CVT) under varying conditions. Specifically, we find that by lowering the growth temperature ($T_{\mathrm{g}}$ $<$ 630$^{\circ}$C), there is a significant increase in both the CDW transition temperature and the residual resistance ratio (RRR) obtained from electrical transport measurements. Using x-ray photoelectron spectroscopy (XPS), we correlate the observed CDW properties with stoichiometry and the nature of defects. In addition, we have optimized a method to grow ultra-high purity 1$T$-VSe$_{2}$ crystals with a CDW transition temperature, $T_{\mathrm{CDW}}$ = (112.7 $\pm$ 0.8) K and maximum residual resistance ratio (RRR) $\approx$ 49, which is the highest reported thus far. This work highlights the sensitivity of the CDW in 1$T$-VSe$_{2}$ to defects and overall stoichiometry, and the importance of controlling the crystal growth conditions of strongly-correlated transition metal dichalcogenides.",2001.08020v2 2020-06-29,Tuning Chern Number in Quantum Anomalous Hall Insulators,"The quantum anomalous Hall (QAH) state is a two-dimensional topological insulating state that has quantized Hall resistance of h/Ce2 and vanishing longitudinal resistance under zero magnetic field, where C is called the Chern number. The QAH effect has been realized in magnetic topological insulators (TIs) and magic-angle twisted bilayer graphene. Despite considerable experimental efforts, the zero magnetic field QAH effect has so far been realized only for C = 1. Here we used molecular beam epitaxy to fabricate magnetic TI multilayers and realized the QAH effect with tunable Chern number C up to 5. The Chern number of these QAH insulators is tuned by varying the magnetic doping concentration or the thickness of the interior magnetic TI layers in the multilayer samples. A theoretical model is developed to understand our experimental observations and establish phase diagrams for QAH insulators with tunable Chern numbers. The realization of QAH insulators with high tunable Chern numbers facilitates the potential applications of dissipationless chiral edge currents in energy-efficient electronic devices and opens opportunities for developing multi-channel quantum computing and higher-capacity chiral circuit interconnects.",2006.16215v3 2021-02-08,"Structural, magnetic, thermodynamic and electrical transport properties of a new compound $\mbox{Pr}_2\mbox{Rh}_{2}\mbox{Ga}$","A new ternary intermetallic compound $\mathrm{Pr_2Rh_2Ga}$ was synthesized by arc-melting and was characterized by powder X-ray diffraction (PXRD), magnetization, heat capacity $\mathrm{C}_p(\textit{T})$, and electrical resistivity $\rho(T)$ measurements. PXRD patterns revealed that $\mathrm{Pr_2Rh_2Ga}$ crystallizes in the $\rm{La_2Ni_3}$-type of orthorhombic structure with the space group $Cmca$. The temperature variation of magnetic susceptibility, $\mathrm {C}_p(\textit{T})$ and $\rho(T)$ confirmed that $\mathrm{Pr_2Rh_2Ga}$ exhibits a ferromagnetic behavior with the transition temperature of 18 K. The estimated Sommerfeld coefficient $\gamma$ = 640 mJ/($\mathrm{Pr.mole.K^2}$) from the $\mathrm {C}_p(\textit{T})$ results in the paramagnetic region just above $T_{C}$~was large in comparison to ordinary metals. In the paramagnetic region $\rho(T)$ data showed a metallic behavior characteristic of electron - phonon scattering. The maximum negative magneto-resistance at high field occurs in the region near the magnetic phase transition temperature. The maximum value of magnetic entropy change ($\rm -\Delta \textit{S}_{M}$) and adiabatic temperature change ($\rm \Delta \textit{T}_{ad}$) are $\rm8.2~J/kg.K$ and $\rm3.6~K$, respectively, around the transition temperature for the change of magnetic field 0-9 T. The calculated refrigerant capacity is $\rm70~J/kg$, and $\rm135~J/kg$ for a change of magnetic field 0-5 T and 0-9 T, respectively. Arrott plot derived from isothermal magnetization and the universal scaling plot by normalizing $\rm -\Delta \textit{S}_{M}$ confirm that the compound undergoes a second order ferromagnetic to paramagnetic phase transition.",2102.04106v2 2021-10-09,Topologically Protected Ferroelectric Domain Wall Memory with Large Readout Current,"The discovery and precise manipulation of atomic-size conductive ferroelectric domain defects, such as geometrically confined walls, offer new opportunities for a wide range of prospective electronic devices, and the so-called walltronics is emerging consequently. Here we demonstrate the highly stable and fatigue-resistant nonvolatile ferroelectric memory device based on deterministic creation and erasure of conductive domain wall geometrically confined inside a topological domain structure. By introducing a pair of delicately designed co-axial electrodes onto the epitaxial BiFeO3 film, one can easily create quadrant center topological polar domain structure. More importantly, a reversible switching of such center topological domain structure between the convergent state with highly conductive confined wall and the divergent state with insulating confined wall can be realized, hence resulting in an apparent resistance change with a large On/Off ratio > 104 and a technically preferred readout current (up to 40 nA). Owing to the topological robustness of the center domain structure, the device exhibits the excellent restoration repeatability over 106 cycles and a long retention over 12 days (> 106 s). This work demonstrates a good example for implementing the exotic polar topologies in high-performance nanoscale devices, and would spur more interest in exploring the rich emerging applications of these exotic topological states.",2110.04530v1 2021-12-05,Insights into Cold Source MOSFETs with Sub-60 mV/decade and Negative Differential Resistance Effect,"To extend the Moores law in the 5 nm node, a large number of two dimensional (2D) materials and devices have been thoroughly researched, among which the cold metals 2H MS2 (M = Nb, Ta) with unique band structures are expected to achieve the sub-60 mV/dec subthreshold swing (SS). The studied cold metal field-effect transistors (CM-FETs) based on the cold metals are capable to fulfill the high-performance (HP) and low-dissipation (LP) goals simultaneously, as required by the International Technology Roadmap for Semiconductors (ITRS). Moreover, gaps of cold metals also enable the CM-FETs to realize negative differential resistance (NDR) effect. Owing to the wide transmission path in the broken gap structure of NbS2/MoS2 heterojunction, the recording 4110 A/m peak current, several orders of magnitude higher than the tunneling current of the Esaki diode, is achieved by NbS2/MoS2 CM-FET. The largest peak-valley ratio (PVR) is obtained by TaS2/MoS2 CM-FET with VGS = -1V at room temperature. Our results claim that the superior on-state current, SS, cut-off frequency and NDR effect can be obtained by CM-FETs simultaneously. The study of CM-FETs provides a practicable solution for state-of-the-art logic device in sub 5 nm node for both more Moore roadmap and more than Moore roadmap applications.",2112.02578v1 2021-12-13,Tunneling Magnetoresistance in Noncollinear Antiferromagnetic Tunnel Junctions,"Antiferromagnetic (AFM) spintronics has emerged as a subfield of spintronics driven by the advantages of antiferromagnets producing no stray fields and exhibiting ultrafast magnetization dynamics. The efficient method to detect an AFM order parameter, known as the N\'eel vector, by electric means is critical to realize concepts of AFM spintronics. Here, we demonstrate that non-collinear AFM metals, such as Mn3Sn, exhibit a momentum dependent spin polarization which can be exploited in AFM tunnel junctions to detect the N\'eel vector. Using first-principles calculations based on density functional theory, we predict a tunneling magnetoresistance (TMR) effect as high as 300% in AFM tunnel junctions with Mn3Sn electrodes, where the junction resistance depends on the relative orientation of their N\'eel vectors and exhibits four non-volatile resistance states. We argue that the spin-split band structure and the related TMR effect can also be realized in other non-collinear AFM metals like Mn3Ge, Mn3Ga, Mn3Pt, and Mn3GaN. Our work provides a robust method for detecting the N\'eel vector in non-collinear antiferromagnets via the TMR effect, which may be useful for their application in AFM spintronic devices.",2112.06568v2 2022-01-26,A new quasi-one-dimensional superconductor parent compound NaMn$_6$Bi$_5$ with lower antiferromagnetic transition temperatures,"Mn-based superconductor is rare and recently reported in quasi-one-dimensional KMn$_6$Bi$_5$ with [Mn$_6$Bi$_5$]-columns under high pressure. Here we report the synthesis, magnetic properties, electrical resistivity, and specific heat capacity of the newly-discovered quasi-one-dimensional NaMn$_6$Bi$_5$ single crystal. Compared with other AMn$_6$Bi$_5$ (A = K, Rb, and Cs), NaMn$_6$Bi$_5$ has larger intra-column Bi-Bi bond length, which may result in the two decoupled antiferromagnetic transitions at 47.3 K and 52.3 K. The relatively lower antiferromagnetic transition temperatures make NaMn$_6$Bi$_5$ a more suitable platform to explore Mn-based superconductors. Anisotropic resistivity and non-Fermi liquid behavior at low temperature are observed. Heat capacity measurement reveals that NaMn$_6$Bi$_5$ has similar Debye temperature with those of AMn$_6$Bi$_5$ (A = K and Rb), whereas the Sommerfeld coefficient is unusually large. Using first-principles calculations, the quite different density of states and an unusual enhancement near the Fermi level are observed for NaMn$_6$Bi$_5$, when compared with those of other AMn$_6$Bi$_5$ (A = K, Rb, and Cs) compounds.",2201.10719v1 2022-09-30,Charge Transport in Ba$_{1-x}$Rb$_{x}$Fe$_{2}$As$_{2}$ Single Crystals,"Recent studies in heavily hole-doped iron-based superconductor RbFe$_2$As$_2$ have suggested the emergence of novel electronic nematicity directed along the Fe-As direction, 45$^\circ$ rotated from the usual nematicity ubiquitously found in BaFe$_2$As$_2$ and related materials. This motivates us to study the physical properties of Ba$_{1-x}$Rb$_{x}$Fe$_{2}$As$_{2}$, details of which remain largely unexplored. Here we report on the normal-state charge transport in Ba$_{1-x}$Rb$_{x}$Fe$_{2}$As$_{2}$ superconductors by using high-quality single crystals in the range of Rb concentration $0.14\le x \le 1.00$. From the systematic measurements of the temperature dependence of electrical resistivity $\rho(T)$, we find a signature of a deviation from the Fermi liquid behavior around the optimal composition, which does not seem related to the antiferromagnetic quantum criticality but has a potential link to hidden nematic quantum criticality. In addition, electron correlations derived from the coefficient of $T^2$ resistivity show a marked increase with Rb content near the heavily hole-doped end, consistent with the putative Mott physics near the $3d^5$ electron configuration in iron-based superconductors.",2209.15526v1 2022-10-14,Physical properties of the layered $f$-electron van der Waals magnet Ce$_2$Te$_5$,"We report a detailed study of the magnetic, transport, and thermodynamic properties of Ce$_2$Te$_5$ single crystals, a layered $f$-electron van der Waals magnet. Four consecutive transitions at $\sim$ 5.2, 2.1, 0.9, and 0.4 K were observed in the $ac$-plane electrical resistivity $\rho$(T), which were further confirmed in specific heat $C_\textrm{p}$(T) measurements. Analysis of the magnetic susceptibility $\chi$(T), the magnetic-field variation of $\rho$(T), and the increase of the first transition temperature ($T_\textrm{c} \sim$ 5.2 K) with applied magnetic field indicates ferromagnetic order, while the decrease of the other transitions with field suggests different states with dominant antiferromagnetic interactions below $T_2 \sim$ 2.1 K, $T_3 \sim$ 0.9 K, and $T_4$ = 0.4 K. Critical behavior analysis around $T_\textrm{c}$ that gives critical exponents $\beta = 0.31(2)$, $\gamma = 0.99(2)$, $\delta = 4.46(1)$, $T_\textrm{c} = 5.32(1)$ K indicates that Ce$_2$Te$_5$ shows a three-dimensional magnetic critical behavior. Moreover, the Hall resistivity $\rho_{\textrm{xy}}$ indicates that Ce$_2$Te$_5$ is a multi-band system with a relatively high electron mobility $\sim 2900$ cm$^2$ V$^{-1}$ s$^{-1}$ near $T_\textrm{c}$, providing further opportunities for future device applications.",2210.07507v1 2023-07-10,Inability of linear axion holographic Gubser-Rocha model to capture all the transport anomalies of strange metals,"In the last decade, motivated by the concept of Planckian relaxation and the possible existence of a quantum critical point in cuprate materials, holographic techniques have been extensively used to tackle the problem of strange metals and high-$T_c$ superconductors. Among the various setups, the linear axion Gubser-Rocha model has often been considered as a promising holographic model for strange metals since endowed with the famous linear in $T$ resistivity property. As fiercely advocated by Phil Anderson, beyond $T$-linear resistivity, there are several additional anomalies unique to the strange metal phase, as for example a Fermi liquid like Hall angle -- the famous problem of the two relaxation scales. In this short note, we show that the linear axion holographic Gubser-Rocha model, which presents a single momentum relaxation time, fails in this respect and therefore is not able to capture the transport phenomenology of strange metals. We prove our statement by means of a direct numerical computation, a previously demonstrated scaling analysis and also a hydrodynamic argument. Finally, we conclude with an optimistic discussion on the possible improvements and generalizations which could lead to a holographic model for strange metals in all their glory.",2307.04433v2 2023-08-20,Pressure-induced double-dome superconductivity in kagome metal CsTi3Bi5,"We present high-pressure resistance measurements up to 40 GPa on recently discovered titanium-based kagome metal CsTi$_3$Bi$_5$. At ambient pressure, CsTi$_3$Bi$_5$ shows no evidence of superconductivity in resistivity and specific heat. By applying pressure, superconductivity emerges and the superconducting transition temperature ${\it T}_{\rm c}$ reaches its first maximum of 1.2 K at $\sim$5 GPa. Then the ${\it T}_{\rm c}$ is suppressed by pressure and cannot be detected around 10 GPa, manifesting as a superconducting dome. Remarkably, upon further increasing pressure above $\sim$13 GPa, another superconducting dome shows up, with the maximum ${\it T}_{\rm c}$ of 0.6 K and ending pressure at $\sim$36 GPa. The variation of ${\it T}_{\rm c}$ displays a clear double-dome shape in the superconducting phase diagram. Our work demonstrates the similarity between CsTi$_3$Bi$_5$ and CsV$_3$Sb$_5$, providing valuable insights into the rich physics of these novel kagome metals.",2308.10129v1 2023-09-20,Highly Conductive RuO$_2$ Thin Films from Novel Facile Aqueous Chemical Solution Deposition,"Ruthenium dioxide (RuO$_2$) thin films were synthesized by Chemical Solution Deposition (CSD) on silicon substrates using only water and acetic acid as solvents. The microstructure, phase-purity, electrical and optical properties as well as the thermal stability of the thin films have been characterized. The microstructure of the thin films strongly depends on the annealing temperature: A smooth thin film was achieved at an annealing temperature of 600$^\circ$C. Higher annealing temperatures (800$^\circ$C) led to radial grain growth and an inhomogeneous thin film. A very low resistivity of 0.89 {\Omega}m was measured for a 220 nm-thick thin film prepared at 600$^\circ$. The resistivity of the thin films increases with temperature, which indicates metallic behavior. Phase-purity of the thin films was confirmed with X-ray Diffraction (XRD) measurements, X-ray Photoelectron Spectroscopy (XPS) and Raman spectroscopy. Transmission and reflectivity measurements indicate that RuO$_2$ efficiently blocks the UV-VIS and IR wavelengths. The optical constants determined via spectroscopic ellipsometry show high absorption in the near-IR region as well as a lower one in the UV-VIS region. The thermal stability was investigated by post-annealing, confirming that the thin films are stable up to 750$^\circ$C in synthetic air.",2310.18319v1 2023-12-31,Structural deformation and irreversible magnetic properties of flexible Co/Pt and Co/Pd thin films,"The successful commercialization of flexible spintronic devices requires a complete understanding of the impact of external strain on the structural, electronic, and magnetic properties of a system. The impact of bending-induced strain on flexible films is studied quite well. However, little is known about the effect of other modes of flexibility, e.g., wrinkling, twisting, peeling, and stretching on the functional properties of flexible films. In this context, perpendicular magnetic anisotropic Co/Pt and Co/Pd thin films are prepared on flexible Kapton substrates, and the impact of the peeling mode is studied in detail. The peeling method generates numerous cracks, and buckling in the thin film, along with localized blister formation imaged by scanning electron microscopy. Further, the resistivity measurement confirms a significant enhancement in sample resistance owing to the severe damage of the films. The structural discontinuities strongly affect the magnetization reversal phenomena as measured by the magneto-optic Kerr effect (MOKE)-based microscopy. The bubble domains got converted to elongated-shaped domains due to several hindrances to the wall motion after strain application. Further, the relaxation measurements reveal that the thermal energy is insufficient to switch the magnetization at a few areas due to their high pinning potential associated with the damages. In contrast to bending-induced strain, here, all the modifications in the functional properties are found to be irreversible in nature.",2401.00482v1 2024-04-09,Thin Accretion disks in GR-MHD simulations,"We review some recent results of general relativistic magnetohydrodynamic (GR-MHD) simulations considering the evolution of geometrically thin disks around a central black hole. Thin disk GR-MHD simulations complement the widely used MAD (Magnetically Arrested Disk) or SANE (Standard And Normal Evolution) approaches of evolving from an initial disk torus. In particular, we discuss the dynamical evolution of the disk, its role in the formation of disk winds or jets, the impact of disk resistivity, and its potential role in generating magnetic flux by an internal disk dynamo. The main characteristics of a thin disk in our approach are the Keplerian rotation of the disk material, which allows to launch disk outflows by the Blandford-Payne magneto-centrifugal effect, in addition to the Blandford-Znajek-driven spine jet from the black hole ergosphere. Thus, for this approach, we neglect disk thermodynamics and radiative effects, concentrating predominantly on the dynamical evolution of the system. Resistive MHD further allows the investigation of physical reconnection and also dynamo action. Magnetic reconnection may generate magnetic islands of plasmoids that are ejected from the disk along with the outflow. We also discussed potential applications of thin disk in explaining the decaying phase of an outburst in black hole X-ray binaries (BH-XRBs). Post-processing of radiation using the simulated dynamical data allows to derive spectra or fluxes, e.g., in the X-ray band, and to derive potential variability characteristics.",2404.06140v1 2002-06-26,Comparative Study of Dense Bulk MgB$_2$ Materials Prepared by Different Methods,"We report on the results of a comparative investigation of highly dense bulk MgB$_2$ samples prepared by three methods: (i) hot deformation; (ii) high pressure sintering; and (iii) mechanical alloying of Mg and B powders with subsequent hot compaction. All types of samples were studied by ac-susceptibility, dc-magnetization and resistivity measurements in magnetic fields up to $\mu_0H=160$ kOe. A small but distinct anisotropy of the upper critical field $H_{c2}^{a,b}/H_{c2}^{c}\sim1.2$ connected with some texture of MgB$_2$ grains was found for the hot deformed samples. The samples prepared by high pressure sintering as well as by mechanical alloying show improved superconducting properties, including high upper critical fields $H_{c2}$ ($\mu_0H_{c2}(0)\sim23$ T), irreversibility fields $H_{irr}$ which are strongly shifted towards higher values $H_{irr}(T)\sim0.8H_{c2}(T)$ and high critical current $J_c$ ($J_c=10^5$ A/cm$^2$ at 20 K and 1 T).",0206513v1 2007-03-06,$t-J$ model one-electron renormalizations: high energy features in photoemission experiments of high-$T_c$ cuprates,"Recent angle-resolved photoemission experiments in hole doped cuprates reported new and interesting high energy features which may be useful for understanding the electronic properties of these materials. Using a perturbative approach, which allows the calculation of dynamical properties in the $t-J$ model, one-electron spectral properties were calculated. A strongly renormalized quasiparticle band near the Fermi surface and incoherent spectra at high energy were obtained. Among different current experimental interpretations, the obtained results are closer to the interpretation given by Pan {\it et al.}\cite{pan}. The self-energy shows large high energy contributions which are responsible for the incoherent structures showed by the spectral functions and the reduction of the quasiparticle weight and bandwidth. According to the calculation, collective charge fluctuations are the main source for the self-energy renormalizations. For testing if the obtained self-energy is compatible with transport measurement the resistivity versus temperature was estimated.",0703152v1 2011-05-31,Multiband Transport in Bilayer Graphene at High Carrier Densities,"We report a multiband transport study of bilayer graphene at high carrier densities. Employing a poly(ethylene)oxide-CsClO$_4$ solid polymer electrolyte gate we demonstrate the filling of the high energy subbands in bilayer graphene samples at carrier densities $|n|\geq2.4\times 10^{13}$ cm$^{-2}$. We observe a sudden increase of resistance and the onset of a second family of Shubnikov de Haas (SdH) oscillations as these high energy subbands are populated. From simultaneous Hall and magnetoresistance measurements together with SdH oscillations in the multiband conduction regime, we deduce the carrier densities and mobilities for the higher energy bands separately and find the mobilities to be at least a factor of two higher than those in the low energy bands.",1106.0035v1 2012-04-30,High Mobility in a Stable Transparent Perovskite Oxide,"We discovered that La-doped BaSnO3 with the perovskite structure has an unprecedentedly high mobility at room temperature while retaining its optical transparency. In single crystals, the mobility reached 320 cm^2(Vs)^-1 at a doping level of 8x10^19 cm^-3, constituting the highest value among wide-band-gap semiconductors. In epitaxial films, the maximum mobility was 70 cm^2(Vs)^-1 at a doping level of 4.4x10^20 cm^-3. We also show that resistance of (Ba,La)SnO3 changes little even after a thermal cycle to 530 Deg. C in air, pointing to an unusual stability of oxygen atoms and great potential for realizing transparent high-frequency, high-power functional devices.",1204.6702v3 2013-01-25,All-Heusler giant-magnetoresistance junctions with matched energy bands and Fermi surfaces,"We present an all-Heusler architecture which could be used as a rational design scheme for achieving high spin-filtering efficiency in the current-perpendicular-to-plane giant magnetoresistance (CPP-GMR) devices. A Co2MnSi/Ni2NiSi/Co2MnSi trilayer stack is chosen as the prototype of such an architecture, of which the electronic structure and magnetotransport properties are systematically investigated by first principles approaches. Almost perfectly matched energy bands and Fermi surfaces between the all-Heusler electrode-spacer pair are found, indicating large interfacial spin-asymmetry, high spin-injection efficiency, and consequently high GMR ratio. Transport calculations further confirms the superiority of the all-Heusler architecture over the conventional Heusler/transition-metal(TM) structure by comparing their transmission coefficients and interfacial resistances of parallel conduction electrons, as well as the macroscopic current-voltage (I-V) characteristics. We suggest future theoretical and experimental efforts in developing novel all-Heusler GMR junctions for the read heads of the next generation high-density hard disk drives (HDDs).",1301.6106v1 2013-05-02,Optimisation of CMOS pixel sensors for high performance vertexing and tracking,"CMOS Pixel Sensors tend to become relevant for a growing spectrum of charged particle detection instruments. This comes mainly from their high granularity and low material budget. However, several potential applications require a higher read-out speed and radiation tolerance than those achieved with available devices based on a 0.35 micrometers feature size technology. This paper shows preliminary test results of new prototype sensors manufactured in a 0.18 micrometers process based on a high resistivity epitaxial layer of sizeable thickness. Grounded on these observed performances, we discuss a development strategy over the coming years to reach a full scale sensor matching the specifications of the upgraded version of the Inner Tracking System (ITS) of the ALICE experiment at CERN, for which a sensitive area of up to about 10 square meters may be equipped with pixel sensors.",1305.0531v2 2014-05-05,High Precision Measurements Using High Frequency Signals,"Generalized lock-in amplifiers use digital cavities with Q-factors as high as 5X10^8. In this letter, we show that generalized lock-in amplifiers can be used to analyze microwave (giga-hertz) signals with a precision of few tens of hertz. We propose that the physical changes in the medium of propagation can be measured precisely by the ultra-high precision measurement of the signal. We provide evidence to our proposition by verifying the Newton's law of cooling by measuring the effect of change in temperature on the phase and amplitude of the signals propagating through two calibrated cables. The technique could be used to precisely measure different physical properties of the propagation medium, for example length, resistance, etc. Real time implementation of the technique can open up new methodologies of in-situ virtual metrology in material design.",1405.0853v1 2014-12-03,High-field thermal transport properties of REBCO coated conductors,"The use of REBCO coated conductors is envisaged for many applications, extending from power cables to high-field magnets. Whatever the case, thermal properties of REBCO tapes play a key role for the stability of superconducting devices. In this work, we present the first study on the longitudinal thermal conductivity ($\kappa$) of REBCO coated conductors in magnetic fields up to 19 T applied both parallelly and perpendicularly to the thermal-current direction. Copper-stabilized tapes from six industrial manufacturers have been investigated. We show that zero-field $\kappa$ of coated conductors can be calculated with an accuracy of $\pm 15%$ from the residual resistivity ratio of the stabilizer and the Cu/non-Cu ratio. Measurements performed at high fields have allowed us to evaluate the consistency of the procedures generally used for estimating in-field $\kappa$ in the framework of the Wiedemann-Franz law from an electrical characterization of the materials. In-field data are intended to provide primary ingredients for the thermal stability analysis of high-temperature superconductor-based magnets.",1412.1328v1 2015-10-19,Simulating feedback from nuclear clusters: the impact of multiple sources,"Nuclear star clusters (NCs) are found to exist in the centres of many galaxies and appear to follow scaling relations similar to those of super-massive black holes. Previous analytical work has suggested that such relations are a consequence of feedback regulated growth. We explore this idea using high resolution hydrodynamical simulations, focusing on the validity of the simplifying assumptions made in analytical models. In particular, we investigate feedback emanating from multiple stellar sources rather than from a single source, as is usually assumed, and show that collisions betweens shells of gas swept up by feedback leads to momentum cancellation and the formation of high density clumps and filaments. This high density material is resistant both to expulsion from the galaxy potential and to disruption by feedback; if it falls back onto the NC, we expect the gas to be available for further star formation or for feeding a central black hole. We also note our results may have implications for the evolution of globular clusters and stellar clusters in high redshift dark matter halos.",1510.05697v1 2016-06-21,Mobility induced unsaturated high linear magnetoresistance in transition-metal monopnictides Weyl semimetals,"Discovery of Weyl fermions in semimetallic tansition-metal monopnictides is a major breakthrough in condensed matter physics. A Weyl semimetal is characterized by the existence of robust Weyl points and unclosed topological surface states in the form of Fermi arc. All the four compounds of the Weyl semimetal transition monopnictide family i.e. NbP, TaP, NbAs and TaAs exhibit extremely high mobility and unsaturated high magnetoresistance (MR). For example, MR values are 8.5x10^5% at 1.85 K for NbP and 1.5x10^5% at 3 K in 9 T for TaAs. NbP also achieves very low value of residual resistivity 0.63 micro-ohm cm at 2 K due to suppression of scattering resulting in ultra-high mobility 5x10^6 cm^2/Vs, Interestingly, we find that the mobility of these compounds play an important role for such a large MR.",1606.06649v1 2017-06-28,First-principles prediction of high-entropy-alloy stability,"High entropy alloys (HEAs) are multicomponent compounds whose high configurational entropy allows them to solidify into a single phase, with a simple crystal lattice structure. Some HEA's exhibit desirable properties, such as high specific strength, ductility, and corrosion resistance, while challenging the scientist to make confident predictions in the face of multiple competing phases. We demonstrate phase stability in the multicomponent alloy system of Cr-Mo-Nb-V, for which some of its binary subsystems are subject to phase separation and complex intermetallic-phase formation. Our first-principles calculation of free energy predicts that the configurational entropy stabilizes a single body-centered cubic (BCC) phase from T = 1,700K up to melting, while precipitation of a complex intermetallic is favored at lower temperatures. We form the compound experimentally and confirm that it forms as a single BCC phase from the melt, but that it transforms reversibly at lower temperatures.",1706.09282v1 2018-05-15,"Unprecedented High Irreversibility Line in Nontoxic Cuprate Superconductor (Cu,C)Ba2Ca3Cu4O11+delta","One of the key factors limiting the high power applications for a type-II superconductor is the irreversibility line Hirr(T) which reflects the very boundary of resistive dissipation in the phase diagram of magnetic field versus temperature. In cuprate family, the Y-, Bi-, Hg- and Tl-based systems have superconducting transition temperatures exceeding the liquid nitrogen boiling temperature (~77K). However, the toxic elements Hg and Tl in the latter two systems strongly constrain the possible applications. The Bi-based (2223) system is nontoxic, but the irreversibility magnetic field is strongly suppressed in the liquid nitrogen temperature region. For this purpose, the best perspective so far is relying on the YBa2Cu3O7 (Tc~90 K) system which is nontoxic and has a relatively high irreversibility magnetic field. Here we report the study of a nontoxic superconductor (Cu,C)Ba2Ca3Cu4O11+{\delta} with Tc = 116K. It is found that the irreversibility magnetic field is unprecedentedly high among all superconductors and it thus provides a great potential of applications in the liquid nitrogen temperature region.",1805.05830v1 2018-11-04,Grain growth in Pt microheaters subjected to high current density under constant power,"When $50$ nm thick Pt microheaters of lateral dimensions $1\times10$ $\mu$m$^2$ are subjected to high electric power their resistance $R$ rises, as expected. Following an initial rise however there is a gradual decrement in $R$ while constant electric power dissipation is maintained. We find that this lowering in $R$ is accompanied by grain growth in the polycrystalline thin Pt film of our heaters. This is confirmed by XRD measurements and SEM imaging. Similar growth in grain size is observed in thin Pt films that are oven-annealed at high temperatures. Thus we argue that maintaining high power dissipation in a microheater has the same effect on its material structure as post-annealing. We observe the in-plane grain size of a $50$ nm thick as-grown Pt film/heater to be $D_\parallel=15$ nm. When post-annealed at a temperature of $T=600^\circ$C for 30 min, $D_\parallel=30$ nm, compared with when electric current is run through a heater we estimate the mean crystalline length to be $D_\parallel=35$ nm.",1811.01434v1 2011-04-15,Structural and Magnetic Phase Transitions in NdCoAsO under High Pressures,"We have investigated structural and magnetic phase transitions under high pressures in a quaternary rare earth transition metal arsenide oxide NdCoAsO compound that is isostructural to high temperature superconductor NdFeAsO. Four-probe electrical resistance measurements carried out in a designer diamond anvil cell show that the ferromagnetic Curie temperature and anti-ferromagnetic Neel temperature increase with an increase in pressure. High pressure x-ray diffraction studies using a synchrotron source show a structural phase transition from a tetragonal phase to a new crystallographic phase at a pressure of 23 GPa at 300 K. The NdCoAsO sample remained anti-ferromagnetic and non-superconducting to temperatures down to 10 K and to the highest pressure achieved in this experiment of 53 GPa. A P-T phase diagram for NdCoAsO is presented to a pressure of 53 GPa and low temperatures of 10 K.",1104.3172v1 2012-06-21,High Performance Single Layered WSe2 p-FETs with Chemically Doped Contacts,"We report high performance p-type field-effect transistors based on single layered (thickness, ~0.7 nm) WSe2 as the active channel with chemically doped source/drain contacts and high-{\kappa} gate dielectrics. The top-gated monolayer transistors exhibit a high effective hole mobility of ~250 cm2/Vs, perfect subthreshold swing of ~60 mV/dec, and ION/IOFF of >10^6 at room temperature. Special attention is given to lowering the contact resistance for hole injection by using high work function Pd contacts along with degenerate surface doping of the contacts by patterned NO2 chemisorption on WSe2. The results here present a promising material system and device architecture for p-type monolayer transistors with excellent characteristics.",1206.4776v1 2020-08-26,Microwave measurements of the high magnetic field vortex motion pinning parameters in Nb$_3$Sn,"The high frequency vortex motion in Nb$_3$Sn was analyzed in this work up to 12 T. We used a dielectric loaded resonator tuned at 15 GHz to evaluate the surface impedance $Z$ of a Nb$_3$Sn bulk sample (24.8 at.\%Sn). From the field induced variation of $Z$, the high frequency vortex parameters (the pinning constant $k_p$, the depinning frequency $\nu_p$ and the flux flow resistivity $\rho_{ff}$) were obtained over a large temperature and field range; their field and temperature dependence were analyzed. Comparison with other superconducting materials shows that high frequency applications in strong magnetic fields are also feasible with Nb$_3$Sn. In the present work, we report the first measurements about the microwave response in Nb$_3$Sn in strong magnetic fields.",2008.11656v3 2021-05-05,High Permittivity Dielectric Field-Plated Vertical (001) $β$-Ga$_2$O$_3$ Schottky Barrier Diode with Surface Breakdown Electric Field of 5.45 MV/cm and BFOM of $>$ 1 GW/cm$^{2}$,"This paper presents vertical (001) oriented $\beta$-Ga$_2$O$_3$ field plated (FP) Schottky barrier diode (SBD) with a novel extreme permittivity dielectric field oxide. A thin drift layer of 1.7 $\mu m$ was used to enable a punch-through (PT) field profile and very low differential specific on-resistance (R$_{on-sp}$) of 0.32 m$\Omega$-cm$^{2}$. The extreme permittivity field plate oxide facilitated the lateral spread of the electric field profile beyond the field plate edge and enabled a breakdown voltage ($V_{br}$) of 687 V. The edge termination efficiency increases from 13.5 $\%$ for non-field plated structure to 63 $\%$ for high permittivity field plate structure. The surface breakdown electric field was extracted to be 5.45 MV/cm at the center of the anode region using TCAD simulations. The high permittivity field plated SBD demonstrated a record high Baliga figure of merit (BFOM) of 1.47 GW/cm$^{2}$ showing the potential of Ga$_2$O$_3$ power devices for multi-kilovolt class applications.",2105.04413v1 2021-06-24,GaN HEMT based high energy particles detection preamplifier,"GaN high electron mobility transistors (HEMT) have gained some foothold in the power electronics industry due to wide frequency bandwidth and power handling. The material offers a wide bandgap and higher critical field strength compared to most wide bandgap semiconductors, resulting in better radiation resistance and theoretically higher speeds as the devices dimensions could be reduced without suffering voltage breakdown. This work consists of the underlying simulation work intended to examine the response of the GaN HEMTs preamlifying circuits for high resolution high energy radiation detectors. The simulation and experimental results illustrate the superior performance of the GaN HEMT in an amplifying circuit. Using a spice model for a commercially available GaN HEMT non distorted output to an input signal of 200 ps was displayed. Real world measurements underscore the fast response of the GaN HEMT with its measured slew rate at approximately 3000 V /{\mu}s a result only 17% lower than the result obtained from the simulation.",2106.12703v1 2022-06-20,Effect of Heat Treatment Mode and Aggressive Media on Mechanical Properties of Porous Polytetrafluoroethylene Membranes Fabricated via Electrospinning,"Electrospinning is a modern alternative to the expanded method for producing porous polytetrafluoroethylene membranes. High strength and relative elongation, as well as the ability to maintain these properties for a long time when exposed to aggressive media at high temperatures, determine the application scope of the electrospun polytetrafluoroethylene membranes. Herein, we report the effect of polytetrafluoroethylene suspension content in the spinning solution, heat treatment mode (quenching and annealing) and aggressive media at high temperatures on the tensile strength and relative elongation of electrospun polytetrafluoroethylene membranes. Membranes fabricated from spinning solutions with 50 to 60 wt % polytetrafluoroethylene suspension content that underwent quenching were characterized by the highest tensile strength and relative elongation. Electrospun polytetrafluoroethylene membranes also demonstrated high chemical resistance to concentrated mineral acids and alkalis, a bipolar aprotic solvent, engine oil and deionized water at 100 deg for 48 hours.",2206.09739v1 2023-01-02,Non-Equilibrium Spark Plasma Reactive Doping Enables Highly Adjustable Metal to Insulator Transitions and Improved Mechanical Stability for VO2,"Although vanadium dioxide (VO2) exhibits the most abrupt metal to insulator transition (MIT) properties near room-temperature, the present regulation of their MIT functionalities is insufficient owing to the high complexity and susception associated with V4+. Herein, we demonstrate a spark plasma assisted reactive sintering (SPARS) approach to simultaneously achieve in situ doping and sintering of VO2 within largely short period (~10 minutes). This enables high convenience and flexibility in regulating the electronic structure of VO2 via dopant elements covering Ti, W, Nb, Mo, Cr and Fe, leading to a wide adjustment in their metal to insulator transition temperature (TMIT) and basic resistivity. Furthermore, the mechanical strengths of the doped-VO2 were meanwhile largely improved via the compositing effect of high melting-point dopant oxide. The high adjustability in MIT properties and improved mechanical properties further paves the way towards practical applications of VO2 in power electronics, thermochromism and infrared camouflage.",2301.00634v1 2024-01-15,High entropy alloys and their affinity to hydrogen: from Cantor to platinum group elements alloys,"Properties of high entropy alloys are currently in the spotlight due to their promising applications. One of the least investigated aspects is the affinity of these alloys to hydrogen, its diffusion and reactions. In this study we apply high-pressure at ambient temperature and investigate stress-induced diffusion of hydrogen into the tructure of high entropy alloys HEA including the famous Cantor alloy as well as less known, but nevertheless important platinum group PGM alloys. By applying X-ray diffraction to samples loaded into diamond anvil cells we perform a comparative investigation of these HEA alloys in Ne and H2 pressure-transmitting media. Surprisingly, even under stresses far exceeding conventional industrial processes both Cantor and PGM alloys show exceptional resistance to hydride formation, on par with widely used industrial grade CuBe alloys. Our observations inspire optimism for practical HEA applications in hydrogen-relevant industry and technology e.g. coatings, etc, particularly those related to transport and storage.",2401.07802v1 2019-10-06,Patterning Sn-based EUV resists with low-energy electrons,"Extreme Ultraviolet (EUV) lithography is the newest technology that will be used in the semiconductor industry for printing circuitry in the sub-20 nm scale. Low-energy electrons (LEEs) produced upon illumination of resist materials with EUV photons (92 eV) play a central role in the formation of the nanopatterns. However, up to now the details of this process are not well understood. In this work, a novel experimental approach that combines Low-Energy Electron Microscopy (LEEM), Electron Energy Loss Spectroscopy (EELS), and Atomic Force Microscopy (AFM) is used to study changes induced by electrons in the 0-40 eV range in thin films of molecular organometallic EUV resists known as tin-oxo cages. LEEM-EELS spectroscopic experiments were used to detect surface charging upon electron exposure and to estimate the electron landing energy. AFM post-exposure analyses revealed that irradiation of the resist with LEEs leads to the densification of the resist layer associated to carbon loss. The same chemical processes that yield densification render the solubility change responsible for the pattern formation in the lithographic application. Remarkably, electrons as low as 1.2 eV are able to induce chemical reactions in the Sn-based resist. Based on the thickness profiles resulting from LEE exposures in the 3-48 mC/cm 2 dose range, a simplified reaction model is proposed where the resist undergoes sequential chemical reactions, yielding first a sparsely cross-linked network, followed by the formation of a denser cross-linked network. This model allows us to estimate a maximum reaction volume on the initial material of 0.15 nm 3 per incident electron in the energy range studied, which means that less than 10 LEEs per molecule on average are needed to turn the material insoluble and thus render a pattern.",1910.02511v1 2010-01-07,Phase change memory technology,"We survey the current state of phase change memory (PCM), a non-volatile solid-state memory technology built around the large electrical contrast between the highly-resistive amorphous and highly-conductive crystalline states in so-called phase change materials. PCM technology has made rapid progress in a short time, having passed older technologies in terms of both sophisticated demonstrations of scaling to small device dimensions, as well as integrated large-array demonstrators with impressive retention, endurance, performance and yield characteristics. We introduce the physics behind PCM technology, assess how its characteristics match up with various potential applications across the memory-storage hierarchy, and discuss its strengths including scalability and rapid switching speed. We then address challenges for the technology, including the design of PCM cells for low RESET current, the need to control device-to-device variability, and undesirable changes in the phase change material that can be induced by the fabrication procedure. We then turn to issues related to operation of PCM devices, including retention, device-to-device thermal crosstalk, endurance, and bias-polarity effects. Several factors that can be expected to enhance PCM in the future are addressed, including Multi-Level Cell technology for PCM (which offers higher density through the use of intermediate resistance states), the role of coding, and possible routes to an ultra-high density PCM technology.",1001.1164v2 2023-04-28,Structural and Optoelectronic Properties of Thin Film LaWN$_3$,"Nitride perovskites are an emerging class of materials that have been predicted to display a range of interesting physics and functional properties, but they are under-explored due to the difficulty of synthesizing oxygen-free nitrides. LaWN3, recently reported as the first oxygen-free nitride perovskite, exhibited polar symmetry and a large piezoelectric coefficient. However, the predicted ferroelectric switching was hindered by large leakage current, which motivates better understanding of its electronic structure and optical properties. Here, we study the structure and optoelectronic properties of thin film LaWN3 in greater detail, employing combinatorial techniques to correlate these properties with cation stoichiometry. We report a two-step synthesis that utilizes a more common RF substrate bias instead of a nitrogen plasma source, yielding nanocrystalline films that are crystallized by ex-situ annealing. We investigate the structure and composition of these films, finding polycrystalline La-rich and highly textured W-rich films. The optical absorption onset and temperature- and magnetic field-dependent resistivity are consistent with semiconducting behavior and are highly sensitive to cation stoichiometry, which may be related to amorphous impurities: metallic W or WNx in W-rich samples and insulating La2O3 in La-rich samples. The fractional magnetoresistance is linear and small, consistent with defect scattering, and a W-rich sample has n-type carriers with high densities and low mobilities. We demonstrate a photoresponse in LaWN3: the resistivity of a La-rich sample is enhanced by 28% at low temperature, likely due to a defect trapping mechanism. The physical properties of LaWN3 are highly sensitive to cation stoichiometry, like many oxide perovskites, which therefore calls for precise composition control to utilize the interesting properties observed in this nitride perovskite.",2305.00098v1 2007-03-12,"Metal-insulator (fermion-boson)-crossover origin of pseudogap phase of cuprates I: anomalous heat conductivity, insulator resistivity boundary, nonlinear entropy","Among all experimental observations of cuprate physics, the metal-insulator-crossover (MIC), seen in the pseudogap (PG) region of the temperature-doping phase diagram of copper-oxides under a strong magnetic field, when the superconductivity is suppressed, is most likely the most intriguing one. Since it was expected that the PG-normal state for these materials, as for conventional superconductors, is conducting. This MIC, revealed in such phenomena as heat conductivity downturn, anomalous Lorentz ratio, insulator resistivity boundary, nonlinear entropy, resistivity temperature upturn, insulating ground state, nematicity- and stripe-phases and Fermi pockets, unambiguously indicates on the insulating normal state, from which the high-temperature superconductivity (HTS) appears. In the present work (article I), we discuss the MIC phenomena mentioned in the title of article. The second work (article II) will be devoted to discussion of other listed above MIC phenomena and also to interpretation of the recent observations in the hidden magnetic order and scanning tunneling microscopy (STM) experiments spin and charge fluctuations as the intra PG and HTS pair ones. We find that all these MIC (called in the literature as non-Fermi liquid) phenomena can be obtained within the Coulomb single boson and single fermion two liquid model, which we recently developed, and the MIC is a crossover of single fermions into those of single bosons. We show that this MIC originates from bosons of Coulomb two liquid model and fermions, whose origin is these bosons. At an increase of doping up to critical value or temperature up to PG boundary temperature, the boson system undegoes bosonic insulator - bosonic metal - fermionic metal transitions.",0703290v3 2009-05-11,"The characteristics of the superconducting and magnetic phases in the polycrystalline samples of ruthenocuprates of nominal compositions RuSr2GdCu2O8, Ru0.98Sr2GdCu2O8 and Ru0.5Sr2GdCu2.5O8-d","The temperature dependencies of the resistivity for the superconducting ruthenocuprates of nominal compositions RuSr2GdCu2O8, Ru0.98Sr2GdCu2O8 and Ru0.5Sr2GdCu2.5O8-d were examined for the magnetic field dependent characteristics of the superconducting transitions. The effect of the insignificant diminishing of the Ru/Cu ratio in parent RuSr2GdCu2O8 was confirmed as relevant for the stabilisation of the superconducting phase. Noted differences in the compared characteristics are interpreted for possible inhomogeneous nucleation of the superconducting phase in the parent ruthenocuprate. The phase anisotropy in RuSr2GdCu2O8 and Ru0.98Sr2GdCu2O8 , in presence of the compounds Ru magnetism, appears to be a cause of a significant softening of the Hc2(T) phase line. An anomalous lowering of the magneto-resistivity was observed in the approx. 10 K range above the onset of the superconducting transition, which may suggest the presence of enhanced superconducting fluctuations in the samples. The positive magnetic field shift of the temperatures, which limit the magneto-resistivity and the specific heat signatures of the magnetic ordered state of the Ru sub-lattice, suggests probing the influence of the ferromagnetic Ru interactions in an effective metallic-like conduction channel present in the samples. Superconducting characteristics of the Ru0.5Sr2GdCu2.5O8-d reveal a significant contribution of the Gd paramagnetic signal at low temperatures, interpreted for the presence of a significant anisotropy of the superconducting phase. It is concluded that the Ru-Cu substituted phases of ruthenocuprates may present an opportunity to investigate the effectively anisotropic superconducting phase despite its comparatively high Tc in the compounds related to the 123-type cuprate superconductor.",0905.1721v4 2014-04-14,"Interplane resistivity of underdoped single crystals (Ba$_{1-x}$K$_x$)Fe$_2$As$_2$, $0 \leq x<0.34$","Temperature-dependent inter-plane resistivity, $\rho _c(T)$, was measured in hole-doped iron-arsenide superconductor (Ba$_{1-x}$K$_x$)Fe$_2$As$_2$ over a doping range from parent compound to optimal doping $T_c\approx 38~K$, $0\leq x \leq 0.34$. Measurements were undertaken on high-quality single crystals grown from FeAs flux. The coupled magnetic/structural transition at $T_{SM}$ leads to clear accelerated decrease of $\rho_c(T)$ on cooling in samples with $T_c <$26~K ($x <0.25$). This decrease in hole-doped material is in notable contrast to an increase in $\rho_c(T)$ in the electron-doped Ba(Fe$_{1-x}$Co$_x$)Fe $_2$As$_2$ and iso-electron substituted BaFe$_2$(As$_{1-x}$P$_x$)$_2$. The $T_{SM}$ decreases very sharply with doping, dropping from $T_s$=71~K to zero on increase of $T_c$ from approximately 25 to 27~K. The $\rho_c(T)$ becomes $T$-linear close to optimal doping. The broad crossover maximum in $\rho_c(T)$, found in the parent BaFe$_2$As$_2$ at around $T_{max} \sim$200~K, shifts to higher temperature $\sim$250~K with doping $x$=0.34. The maximum shows clear correlation with the broad crossover feature found in the temperature-dependent in-plane resistivity $\rho_a(T)$. The doping evolution of $T_{max}$ in (Ba$_{1-x}$K$_x$)Fe$_2$As$_2$ is in notable contrast with both rapid suppression of $T_{max}$ found in Ba(Fe$_{1-x}TM_x$)$_2$As$_2$ ($TM$=Co,Rh,Ni,Pd) and its rapid increase BaFe$_2$(As$_{1-x}$P$_x$)$_2$. This observation suggest that pseudogap features are much stronger in hole-doped than in electron-doped iron-based superconductors, revealing significant electron-hole doping asymmetry similar to the cuprates. This paper replaces: cond-mat:1106.0533.",1404.3664v1 2016-02-02,Field-insensitive heavy fermion features and phase transition in the caged-structure quasi-skutterudite Sm$_3$Ru$_4$Ge$_{13}$,"The robust field-insensitive heavy fermion features in Sm$_3$Ru$_4$Ge$_{13}$ and the magnetic phase transition at $T_N \approx$ 5~K are studied using magnetization $M(T)$, specific heat $C_p(T)$, resistivity $\rho(T)$ and thermal conductivity $\kappa_T(T)$. The average crystal structure of Sm$_3$Ru$_4$Ge$_{13}$ conforms to the cubic space group $Pm\bar{3}n$ however, signatures of subtle structural distortions are obtained from the x ray data. The magnetic susceptibility, $\chi(T)$, follows a modified Curie-Weiss law indicating the presence of crystal fields of Sm$^{3+}$ and the significance of van Vleck terms. No sign of ferromagnetism is observed in $M(H)$ of Sm$_3$Ru$_4$Ge$_{13}$ which yields only 0.025~$\mu_\mathrm{B}$/f.u.-Sm at 2~K, 7~T. The Sommerfeld coefficient, $\gamma \approx$ 220~mJ/mol-Sm K$^2$, estimated from the analysis of low temperature specific heat suggests the formation of heavy quasi particles at low temperature. Though a ln$T$ dependence of $\rho(T)$ is observed till 60~K, the resistivity behavior is accounted for by assuming a two-band model for activated behavior of charge carriers. The field scans of resistivity, $\rho(H)$, below $T_N$ display significant nonlinearity while those above the $T_N$ are more metal-like. Low values of thermal conductivity, $\kappa_T(T)$, are observed in Sm$_3$Ru$_4$Ge$_{13}$ however, displaying an anomaly at $T_N$ which signifies magnetoelastic coupling. A fairly high value of Seebeck coefficient, $S \approx$ 40~$\mu$V/K is observed at 300~K. We identify Sm$_3$Ru$_4$Ge$_{13}$ as a low charge carrier density system with unusual field-insensitive heavy fermion features very similar to the filled skutterudites.",1602.00957v1 2018-03-11,Anomalous metamagnetism in the low carrier density Kondo lattice YbRh3Si7,"We report complex metamagnetic transitions in single crystals of the new low carrier Kondo antiferromagnet YbRh3Si7. Electrical transport, magnetization, and specific heat measurements reveal antiferromagnetic order at T_N = 7.5 K. Neutron diffraction measurements show that the magnetic ground state of YbRh3Si7 is a collinear antiferromagnet where the moments are aligned in the ab plane. With such an ordered state, no metamagnetic transitions are expected when a magnetic field is applied along the c axis. It is therefore surprising that high field magnetization, torque, and resistivity measurements with H||c reveal two metamagnetic transitions at mu_0H_1 = 6.7 T and mu_0H_2 = 21 T. When the field is tilted away from the c axis, towards the ab plane, both metamagnetic transitions are shifted to higher fields. The first metamagnetic transition leads to an abrupt increase in the electrical resistivity, while the second transition is accompanied by a dramatic reduction in the electrical resistivity. Thus, the magnetic and electronic degrees of freedom in YbRh3Si7 are strongly coupled. We discuss the origin of the anomalous metamagnetism and conclude that it is related to competition between crystal electric field anisotropy and anisotropic exchange interactions.",1803.04013v2 2021-01-28,Direct Opto-Electronic Imaging of 2D Semiconductor - 3D Metal Buried Interfaces,"The semiconductor-metal junction is one of the most critical factors for high performance electronic devices. In two-dimensional (2D) semiconductor devices, minimizing the voltage drop at this junction is particularly challenging and important. Despite numerous studies concerning contact resistance in 2D semiconductors, the exact nature of the buried interface under a three-dimensional (3D) metal remains unclear. Herein, we report the direct measurement of electrical and optical responses of 2D semiconductor-metal buried interfaces using a recently developed metal-assisted transfer technique to expose the buried interface which is then directly investigated using scanning probe techniques. We characterize the spatially varying electronic and optical properties of this buried interface with < 20 nm resolution. To be specific, potential, conductance and photoluminescence at the buried metal/MoS$_2$ interface are correlated as a function of a variety of metal deposition conditions as well as the type of metal contacts. We observe that direct evaporation of Au on MoS$_2$ induces a large strain of ~5% in the MoS$_2$ which, coupled with charge transfer, leads to degenerate doping of the MoS$_2$ underneath the contact. These factors lead to improvement of contact resistance to record values of 138 kohm-um, as measured using local conductance probes. This approach was adopted to characterize MoS$_2$-In/Au alloy interfaces, demonstrating contact resistance as low as 63 kohm-um. Our results highlight that the MoS$_2$/Metal interface is sensitive to device fabrication methods, and provides a universal strategy to characterize buried contact interfaces involving 2D semiconductors.",2101.12203v1 2016-09-12,"Magnetic, specific heat and electrical transport properties of Frank-Kasper cage compounds RTM$_2$Al$_{20}$ [R = Eu,Gd and La ; TM = V,Ti]","Single crystals of Frank-Kasper compounds RTM$_2$Al$_{20}$ (R = Eu, Gd and La; TM = V and Ti) were grown by self-flux method and their physical properties were investigated through magnetization ($M$), magnetic susceptibility ($\chi$), specific heat ($C_P$) and electrical resistivity ($\rho$) measurements. Powder x-ray diffraction studies and structural analysis showed that these compounds crystallize in the cubic crystal structure with the space group $Fd\overline{3}m$. The magnetic susceptibility for the compounds EuTi$_2$Al$_{20}$ and GdTi$_2$Al$_{20}$ showed a sudden jump below the N{\'e}el temperature $T_N$ indicative of plausible double magnetic transition. Specific heat ($C_P$) and electrical resistivity ($\rho$) measurements also confirm the first-order magnetic transition (FOMT) and possible double magnetic transitions. Temperature variation of heat capacity showed a sharp phase transition and huge $C_P$ value for the (Eu/Gd)Ti$_2$Al$_{20}$ compounds Full width at half-maximum (FWHM) $<$ 0.2 K) which is reminiscent of a first-order phase transition and a unique attribute among RTM$_2$Al$_{20}$ compounds. We observed clear anomaly between heating and cooling cycle in temperature-time relaxation curve for the compounds GdTi$_2$Al$_{20}$ (2.38 $K$) and EuTi$_2$Al$_{20}$ (3.2 $K$) which is indicating a thermal arrest due to the latent heat. The temperature variation of $S_{mag}$ for GdTi$_2$Al$_{20}$ saturates to a value $0.95R\ln8$ while the other magnetic systems exhibited still lower entropy saturation values in the high temperature limit. Resistivity measurements showed that all the samples behave as normal Fermi liquid type compounds and $\rho(T)$ due to electron-phonon scattering follows Bloch-Gr$\ddot{\textrm u}$neisen-Mott relation in the paramagnetic region.",1609.03458v1 2019-01-25,Insulator-like behavior coexisting with metallic electronic structure in strained FeSe thin films grown by molecular beam epitaxy,"This paper reports that ~10-nm-thick FeSe thin films exhibit insulator-like behavior in terms of the temperature dependence of their electrical resistivity even though bulk FeSe has a metallic electronic structure that has been confirmed by photoemission spectroscopy and first-principles calculations. This apparent contradiction is explained by potential barriers formed in the conduction band. Very thin FeSe epitaxial films with various [Fe]/[Se] were fabricated by molecular beam epitaxy and classified into two groups with respect to lattice strain and electrical properties. Lattice parameter a increased and lattice parameter c decreased with increasing [Fe]/[Se] up to 1.1 and then a levelled off and c began to decrease at higher [Fe]/[Se]. Consequently, the FeSe films had the most strained lattice when [Fe]/[Se] was 1.1, but these films had the best quality with respect to crystallinity and surface flatness. All the FeSe films with [Fe]/[Se] of 0.8-1.9 exhibited insulator-like behavior, but the temperature dependences of their electrical resistivities exhibited different activation energies Ea between the Se-rich and Fe-rich regions; i.e., Ea were small (a few meV) up to [Fe]/[Se]=1.1 but jumped up to ~25 meV at higher [Fe]/[Se]. The film with [Fe]/[Se]=1.1 had the smallest Ea of 1.1 meV and exhibited an insulator-superconducting transition at 35 K with zero resistance under gate bias. The large Ea of the Fe-rich films was attributed to the unusual lattice strain with tensile in-plane and relaxed out-of-plane strains. The large Ea of films with [Fe]/[Se]>1.1 resulted in low mobility with a high potential barrier of ~50 meV in the conduction band for percolation carrier conduction compared with that of the [Fe]/[Se]=1.1 film (~17 meV). Therefore, the Fe-rich films exhibited remarkable insulator-like behavior similar to a semiconductor despite their metallic electronic structure.",1901.08780v1 2019-10-23,Persistent Insulator: Avoidance of Metallization at Megabar Pressures in Strongly Spin-Orbit-Coupled Sr2IrO4,"It is commonly anticipated that an insulating state collapses in favor of an emergent metallic state at high pressures as the unit cell shrinks and the electronic bandwidth broadens to fill the insulating energy band gap. Here we report a rare insulating state that persists up to at least 185 GPa in the antiferromagnetic iridate Sr2IrO4, which is the archetypical spin-orbit-driven Jeff = 1/2 insulator. This study shows the electrical resistance of single-crystal Sr2IrO4 initially decreases with applied pressure, reaches a minimum in the range, 32 - 38 GPa, then abruptly rises to fully recover the insulating state with further pressure increases up to 185 GPa. Our synchrotron x-ray diffraction and Raman scattering data show the onset of the rapid increase in resistance is accompanied by a structural phase transition from the native tetragonal I41/acd phase to an orthorhombic Pbca phase (with much reduced symmetry) at 40.6 GPa. The clear-cut correspondence of these two anomalies is key to understanding the stability of the insulating state at megabar pressures: Pressure-induced, severe structural distortions prevent the expected metallization, despite the 26% volume compression attained at the highest pressure accessed in this study. Moreover, the resistance of Sr2IrO4 remains stable while the applied pressure is tripled from 61 GPa to 185 GPa. These results suggest that a novel type of electronic Coulomb correlation compensates the anticipated band broadening in strongly spin-orbit-coupled materials at megabar pressures.",1910.10291v1 2020-06-19,Synthesis and study of highly dense and smooth TiN thin films,"This study aims towards a systematic reciprocity of the tunable synthesis parameters - partial pressure of N$_2$ gas, ion energy (\Ei) and Ti interface in TiN thin film samples deposited using ion beam sputtering at ambient temperature (300\,K). At the optimum partial pressure of N$_2$ gas, samples were prepared with or without Ti interface at \Ei~=~1.0 or 0.5\,keV. They were characterized using x-ray reflectivity (XRR) to deduce thickness, roughness and density. The roughness of TiN thin films was found to be below 1\,nm, when deposited at the lower \Ei~of 0.5\,keV and when interfaced with a layer of Ti. Under these conditions, the density of TiN sample reaches to 5.80($\pm$0.03)\,g~cm$^{-3}$, a value highest hitherto for any TiN sample. X-ray diffraction and electrical resistivity measurements were performed. It was found that the cumulative effect of the reduction in \Ei~from 1.0 to 0.5\,keV and the addition of Ti interface favors (111) oriented growth leading to dense and smooth TiN films and a substantial reduction in the electrical resistivity. The reduction in \Ei~has been attributed to the surface kinetics mechanism (simulated using SRIM) where the available energy of the sputtered species (\Esp) leaving the target at \Ei~= 0.5\,keV is the optimum value favoring the growth of defects free homogeneously distributed films. The electronic structure of samples was probed using N K-edge absorption spectroscopy and the information about the crystal field and spin-orbit splitting confirmed TiN phase formation. In essence, through this work, we demonstrate the role of \Esp~and Ti interface in achieving highly dense and smooth TiN thin films with low resistivity without the need of a high temperature or substrate biasing during the thin film deposition process.",2006.11055v1 2020-12-31,Room-temperature superconductivity in an artificial 2D Mott-insulating square lattice and its advanced condensed phase that generates a low-loss current in the atmosphere: A possible perpetual motion machine,"A 2D metallic phononic crystal (PnC), which is fabricated by drilling periodic holes in a suspended niobium (Nb) film, is repeatedly cooled and warmed in the temperature range of 2--300 K. During the first five temperature cycles, the resistance of the metallic PnC gradually increases in accordance with the Friedel sum rule, indicating that narrow Nb bridges between adjacent thru-holes are converted into $d$-orbital-filled Mott insulators. The consequent 2D Mott-insulating square lattice is a crystallographic analog of a copper oxide layer in high-temperature superconductors such as YBCO and BSCCO. Subsequent temperature cycles of the thus produced ideal Hubbard crystal realize zero resistance at 60 K, and the zero-resistance state remains up to 300 K, being retained in the atmosphere (i.e., at room temperature, in a terrestrial magnetic field, and under atmospheric pressure). The necessity of the latter temperature cycles remains unclear in this study; however, a possible transition mechanism involving the combined Josephson and charging effects is discussed. The critical current and critical field of the room-temperature superconductor (RTSC) are $I_{C}$ = 18.8 mA and $\mu_{0}H_{\perp}$ = 12 T, respectively. Once a large current exceeding $I_{C}$ is applied to the RTSC, some of the $d$ electrons are forced out, and a special interface consisting of the p-type semiconducting and superconducting states is formed. Carriers diffuse because of the nonequilibrium charge concentration, but they are Andreev-reflected back. In the reversible, thermally isolated system, the entropy never increases, and a simple experiment confirms a low-loss current generated from the interface spontaneously. That is, this study challenges the forbidden perpetual motion machine which can be a solution to the World energy crisis.",2012.15858v1 2021-03-25,Distinct quantum anomalous Hall ground states induced by magnetic disorders,"The quantum anomalous Hall (QAH) effect in magnetic topological insulator (TI) represents a new state of matter originated from the interplay between topology and magnetism. The defining characteristics of the QAH ground state are the quantized Hall resistivity ($\rho_{yx}$) and vanishing longitudinal resistivity ($\rho_{xx}$) in the absence of external magnetic field. A fundamental question concerning the QAH effect is whether it is merely a zero-magnetic-field quantum Hall (QH) effect, or if it can host unique quantum phases and phase transitions that are unavailable elsewhere. The most dramatic departure of the QAH systems from other QH systems lies in the strong magnetic disorders that induce spatially random magnetization. Because disorder and magnetism play pivotal roles in the phase diagram of two-dimensional electron systems, the high degree of magnetic disorders in QAH systems may create novel phases and quantum critical phenomena. In this work, we perform systematic transport studies of a series of magnetic TIs with varied strength of magnetic disorders. We find that the ground state of QAH effect can be categorized into two distinct classes: the QAH insulator and anomalous Hall (AH) insulator phases, as the zero-magnetic-field counterparts of the QH liquid and Hall insulator in the QH systems. In the low disorder limit of the QAH insulator regime, we observe a universal quantized longitudinal resistance $\rho_{xx} = h/e^{2}$ at the coercive field. In the AH insulator regime, we find that a magnetic field can drive it to the QAH insulator phase through a quantum critical point with distinct scaling behaviors from that in the QH phase transition. We propose that the transmission between chiral edge states at domain boundaries, tunable by disorder and magnetic fields, is the key for determining the QAH ground state.",2103.13783v1 2021-04-08,"Extremely large magnetoresistance in the ""ordinary"" metal ReO3","The extremely large magnetoresistance (XMR) observed in many topologically nontrivial and trivial semimetals has attracted much attention in relation to its underlying physical mechanism. In this paper, by combining the band structure and Fermi surface (FS) calculations with the Hall resistivity and de Haas-Van Alphen (dHvA) oscillation measurements, we studied the anisotropy of magnetoresistance (MR) of ReO$_3$ with a simple cubic structure, an ""ordinary"" nonmagnetic metal considered previously. We found that ReO$_3$ exhibits almost all the characteristics of XMR semimetals: the nearly quadratic field dependence of MR, a field-induced upturn in resistivity followed by a plateau at low temperatures, high mobilities of charge carriers. It was found that for magnetic field \emph{H} applied along the \emph{c} axis, the MR exhibits an unsaturated \emph{H}$^{1.75}$ dependence, which was argued to arise from the complete carrier compensation supported by the Hall resistivity measurements. For \emph{H} applied along the direction of 15$^\circ$ relative to the \emph{c} axis, an unsaturated \emph{H}$^{1.90}$ dependence of MR up to 9.43~$\times$~$10^3$$\%$ at 10~K and 9~T was observed, which was explained by the existence of electron open orbits extending along the $k_{x}$ direction. Two mechanisms responsible for XMR observed usually in the semimetals occur also in the simple metal ReO$_3$ due to its peculiar FS (two closed electron pockets and one open electron pocket), once again indicating that the details of FS topology are a key factor for the observed XMR in materials.",2104.03799v1 2021-05-06,A strange metal in a bosonic system,"Fermi liquid theory forms the basis for our understanding of the majority of metals, which is manifested in the description of transport properties that the electrical resistivity goes as temperature squared in the limit of zero temperature. However, the observations of strange metal states in various quantum materials, notably high-temperature superconductors, bring this spectacularly successful theoretical framework into crisis. When electron scattering rate 1/{\tau} hits its limit, kBT/{\hbar} where {\hbar} is the reduced Planck's constant, T represents absolute temperature and kB denotes Boltzmann's constant, Planckian dissipation occurs and lends strange metals a surprising link to black holes, gravity, and quantum information theory. Here, we show the characteristic signature of strange metallicity arising unprecedentedly in a bosonic system. Our nanopatterned YBa2Cu3O7-{\delta}(YBCO) film arrays reveal T-linear resistance as well as B-linear magnetoresistance over an extended temperature and magnetic field range in a quantum critical region in the phase diagram. Moreover, the slope of the T-linear resistance {\alpha}_cp appears bounded by {\alpha}_cp {\approx} h/2e^2 [1/T]_c^onset where T_c^onset is the temperature at which Cooper pairs form, intimating a common scale-invariant transport mechanism corresponding to Planckian dissipation.In contrast to fermionic systems where the temperature and magnetic field dependent scattering rates combine in quadrature of {\hbar}/{\tau} {\approx} {\sqrt} (((k_B T)^2+({\mu}_B B)^2)), both terms linearly combine in the present bosonic system, i.e. {\hbar}/{\tau} {\approx} (k_B T+[{\gamma}{\mu}]_B B), where {\gamma} is a constant. By extending the reach of strange metal phenomenology to a bosonic system, our results suggest that there is a fundamental principle governing their transport which transcends particle statistics.",2105.02654v1 2021-09-22,Discs and outflows in the early phases of massive star formation: influence of magnetic fields and ambipolar diffusion,"We study mass accretion and ejection in the vicinity of massive star forming cores using high-resolution (5 au) 3D AMR numerical simulations. We investigate the mechanisms at the origin of outflows and characterise the properties of the disc forming around massive protostars. We include both protostellar radiative feedback via PMS evolutionary tracks and magnetic ambipolar diffusion. We studied 3 different cases: purely hydrodynamical, ideal MHD, and ambipolar diffusion. In the resistive models, we investigate the effects the initial amplitude of both magnetic field and rotation have on the properties of the massive protostellar system. We use simple criteria to identify the outflow and disc material and follow their evolution as the central star accretes mass up to 20 solar mass. The outflow is completely different when magnetic fields are introduced, so that magnetic processes are the main driver of the outflow up to stellar masses of ~20 solar mass. The disc properties depend on the physics included. The disc formed in the ideal and resistive runs show opposite properties in terms of plasma beta and of magnetic fields topology. While the disc in the ideal case is dominated by the magnetic pressure and the toroidal magnetic fields, the one formed in the resistive runs is dominated by the thermal pressure and has essentially vertical magnetic fields in the inner regions (R<200 au). We find that magnetic processes dominate the early evolution of massive protostellar systems (<20 solar mass) and shapes the accretion/ejection as well as the disc formation. Ambipolar diffusion is mainly at work at disc scales and regulates its properties. Our finding for the outflow and disc properties are reminiscent of low-mass star formation, suggesting that accretion and ejection in young massive and low-mass protostars are regulated by the same physical processes at the early stages.",2109.10580v1 2022-05-03,The Resistive Nature of Decomposing Interfaces of Solid Electrolytes with Alkali Metal Electrodes,"A crucial ingredient in lithium (Li) and sodium (Na)-ion batteries (LIBs and NIBs) is the electrolytes. The use of Li-metal (Na-metal) as anode in liquid electrolyte LIBs (NIBs) is constrained by several issues including thermal runway and flammability, electrolyte leakage, and limited chemical stability. Considerable effort has been devoted toward the development of solid electrolytes (SEs) and all-solid-state batteries, which are presumed to mitigate some of the issues of Li-metal(Na-metal) in contact with flammable liquid electrolytes. However, most SEs, such as Li$_3$PS$_4$, Li$_6$PS$_5$Cl and Na$_3$PS$_4$ readily decompose against the highly reducing Li-metal and Na-metal anodes. Using first-principles calculations we elucidate the stability of more than 20 solid$||$solid interfaces formed between the decomposition products of Li$_3$PS$_4$, Li$_6$PS$_5$Cl (and Na$_3$PS$_4$) against the Li-metal (Na-metal) electrode. We suggest that the work of adhesion needed to form a hetereogenous interfaces is an important descriptor to quantify the stability of interfaces. Subsequently, we clarify the atomistic origins of the resistance to Li-ion transport at interfaces of the Li-metal anode and selected decomposition products (Li$_3$P, Li$_2$S} and LiCl) of SEs, via a high-fidelity machine learned potential (MLP). Utilising an MLP enables nano-second-long molecular dynamics simulations on `large' interface models (here with 8320 atoms), but with similar accuracy to first-principles approaches. Our simulations demonstrate that the interfaces formed between Li-metal and argyrodite (e.g., Li$_6$PS$_5$Cl) decomposition products are resistive to Li-ion transport. The implications of this study are important since binary compounds are commonly found in the vicinity of Li(Na)-metal upon chemical and/or electrochemical decomposition of ternary and quaternary SEs.",2205.01264v1 2015-09-22,Stability and scalability of piezoelectric flags,"We investigate the effect of piezoelectric (PZT) material on the flutter speed, vibration mode and frequency, and energy harvesting power and efficiency of a flexible flag in various fluids. We develop a fully coupled fluid-solid-electric model by combining the inviscid vortex sheet model with a linear electro-mechanical coupling model. A resistance only circuit and a resonant resistance-inductance (RL) circuit are considered. For a purely resistive circuit, an increased electro-mechanical coupling factor results in an increased flutter speed, vibration frequency, averaged electric power and efficiency. A consistent optimal resistance is found that maximizes the flutter speed and the energy harvesting power. For a resonant RL circuit, by tuning the inductance to match the circuit frequency to the flag's vibration frequency, the flutter speed can be greatly decreased, and a larger averaged power and efficiency are obtained. We also consider a model scale set-up with several commonly used commercial materials for operating in air and water. Typical ranges of dimensionless parameters are obtained for four types of material that span a wide range of solid density and rigidity values. We find that the resistance only circuit is more effective when the flag is placed in a lighter fluid (e.g. air), while the RL circuit is able to reduce the flutter speed when the flag is placed in a heavier fluid (e.g. water).",1509.06726v1 2019-09-25,Phonon Scattering at Kinks in Suspended Graphene,"Recent experiments have shown surprisingly large thermal time constants in suspended graphene ranging from 10 to 100 ns in drums with a diameter ranging from 2 to 7 microns. The large time constants and their scaling with diameter points towards a thermal resistance at the edge of the drum. However, an explanation of the microscopic origin of this resistance is lacking. Here, we show how phonon scattering at a kink in the graphene, e.g. formed by sidewall adhesion at the edge of the suspended membrane, can cause a large thermal time constant. This kink strongly limits the fraction of flexural phonons that cross the suspended graphene edge, which causes a thermal interface resistance at its boundary. Our model predicts thermal time constants that are of the same order of magnitude as experimental data, and shows a similar dependence on the circumference. Furthermore, the model predicts the relative in-plane and out-of-plane phonon contributions to graphene's thermal expansion force, in agreement with experiments. We thus show, that in contrast to conventional thermal (Kapitza) resistance which occurs between two different materials, in 2D materials another type of thermal interface resistance can be geometrically induced in a single material.",1909.11615v1 2019-12-24,Tunable Contact Resistance in Transition Metal Dichalcogenide Lateral Heterojunctions,"Contact resistance of semiconducting transition metal dichalcogenides has been shown to decrease in lateral heterojunctions formed with their metallic phases but its origins remain elusive. Here we combine first principles and quantum transport calculations to rationalize the contact resistance of these structures in terms of phase, composition (WTe2, MoTe2, WSe2, and MoSe2), and length of the channel. We find that charge injection in metallic 1T'-WTe2/1T'-MoTe2 junctions is nearly ideal as electrode Bloch states remain delocalized through the channel. Mixtures of 1T' selenides and tellurides depart from this scenario due to the momentum mismatch between states in the lead and channel. In semiconducting channels, the large Schottky barriers degrade the electrical contacts. Around band edges, contact resistance values are about an order of magnitude lower than those obtained experimentally suggesting that doping and phase-engineering could be employed to overcome this issue. We predict that transport regime in these junctions shifts from thermionic emission to tunneling for channels shorter than 3 nm at room temperature. We also discuss the presence of states at the metal/semiconductor interfaces. By underpinning mechanisms to control the contact resistance in heterogeneous two-dimensional materials, this work proves valuable towards the development of devices suitable for optoelectronics and phase-change materials applications.",1912.13500v1 2022-05-12,Chromium-Doped Bismuth Antimony Telluride for Future Quantum Hall Resistance Standards,"Since 2017, epitaxial graphene has been the base material for the US national standard for resistance. A future avenue of research within electrical metrology is to remove the need for strong magnetic fields, as is currently the case for devices exhibiting the quantum Hall effect. The quantum Hall effect is just one of many research endeavours that revolve around recent quantum physical phenomena like composite fermions, charge density waves, and topological properties [1-2]. New materials, like magnetically doped topological insulators (MTIs), offer access to the quantum anomalous Hall effect, which in its ideal form, could become a future resistance standard needing only a small permanent magnet to activate a quantized resistance value [3-5]. Furthermore, these devices could operate at zero-field for measurements, making the dissemination of the ohm more economical and portable. Here we present results on precision measurements of the h/e2 quantized plateau of Cr-Doped (BixSb1-x)2Te3 and give them context by comparing them to modern graphene-based resistance standards. Ultimately, MTI-based devices could be combined in a single system with magnetic-field-averse Josephson voltage standards to obtain an alternative quantum current standard.",2205.06077v1 2024-01-23,Wide-range resistivity characterization of semiconductors with terahertz time-domain spectroscopy,"Resistivity is one of the most important characteristics in the semiconductor industry. The most common way to measure resistivity is the four-point probe method, which requires physical contact with the material under test. Terahertz time domain spectroscopy, a fast and non-destructive measurement method, is already well established in the characterization of dielectrics. In this work, we demonstrate the potential of two Drude model-based approaches to extract resistivity values from terahertz time-domain spectroscopy measurements of silicon in a wide range from about 10$^{-3}$ $\Omega$cm to 10$^{2}$ $\Omega$cm. One method is an analytical approach and the other is an optimization approach. Four-point probe measurements are used as a reference. In addition, the spatial resistivity distribution is imaged by X-Y scanning of the samples to detect inhomogeneities in the doping distribution.",2401.12787v1 2005-04-13,Growth Mechanisms and Oxidation-Resistance of Gold-Coated Iron Nanoparticles,"We report the chemical synthesis of Fe-core/Au-shell nanoparticles by a reverse micelle method, and the investigation of their growth mechanisms and oxidation-resistant characteristics. The core-shell structure and the presence of the Fe & Au phases have been confirmed by transmission electron microscopy, energy dispersive spectroscopy, X-ray diffraction, Mossbauer spectroscopy, and inductively coupled plasma techniques. Additionally, atomic-resolution Z-contrast imaging and electron energy loss spectroscopy (EELS) in a scanning transmission electron microscope (STEM) have been used to study details of the growth processes. The Au-shell grows by nucleating on the Fe-core surface before coalescing. The magnetic moments of such nanoparticles, in the loose powder form, decrease over time due to oxidation. The less than ideal oxidation-resistance of the Au shell may have been caused by the rough Au surfaces. However, in the pressed pellet form, electrical transport measurements show that the particles are fairly stable, as the resistance of the pellet does not change appreciably over time.",0504314v1 2005-11-14,Reproducible Low Contact Resistance in Rubrene Single-Crystal Field-Effect Transistors with Nickel Source and Drain Electrodes,"We have investigated the contact resistance of rubrene single-crystal field-effect transistors (FETs) with Nickel electrodes by performing scaling experiments on devices with channel length ranging from 200 nm up to 300 $\mu$m. We find that the contact resistance can be as low as 100 $\Omega$cm with narrowly spread fluctuations. For comparison, we have also performed scaling experiments on similar Gold-contacted devices, and found that the reproducibility of FETs with Nickel electrodes is largely superior. These results indicate that Nickel is a very promising electrode material for the reproducible fabrication of low resistance contacts in organic FETs.",0511333v1 2005-11-23,Tuning the conductance of single-walled carbon nanotubes by ion irradiation in the Anderson localization regime,"Carbon nanotubes are a good realization of one-dimensional crystals where basic science and potential nanodevice applications merge. Defects are known to modify the electrical resistance of carbon nanotubes. They can be present in as-grown carbon nanotubes, but controlling externally their density opens a path towards the tuning of the nanotube electronic characteristics. In this work consecutive Ar+ irradiation doses are applied to single-walled nanotubes (SWNTs) producing a uniform density of defects. After each dose, the room temperature resistance versus SWNT-length [R(L)] along the nanotube is measured. Our data show an exponential dependence of R(L) indicating that the system is within the strong Anderson localization regime. Theoretical simulations demonstrate that mainly di-vacancies contribute to the resistance increase induced by irradiation and that just a 0.03% of di-vacancies produces an increase of three orders of magnitude in the resistance of a 400 nm SWNT length.",0511585v1 2009-07-13,Enhanced Room Temperature Coefficient of Resistance and Magneto-resistance of Ag-added La0.7Ca0.3-xBaxMnO3 Composites,"In this paper we report an enhanced temperature coefficient of resistance (TCR) close to room temperature in La0.7Ca0.3-xBaxMnO3 + Agy (x = 0.10, 0.15 and y = 0.0 to 0.40) (LCBMO+Ag) composite manganites. The observed enhancement of TCR is attributed to the grain growth and opening of new conducting channels in the composites. Ag addition has also been found to enhance intra-granular magneto-resistance. Inter-granular MR, however, is seen to decrease with Ag addition. The enhanced TCR and MR at / near room temperature open up the possibility of the use of such materials as infrared bolometric and magnetic field sensors respectively.",0907.2134v2 2009-09-21,Spin torque and charge resistance of ferromagnetic semiconductor $2π$ and $π$ domain walls,"Charge resistance and spin torque are generated by coherent carrier transport through ferromagnetic 360 degree domain walls, although they follow qualitatively different trends than for 180 degree domain walls. The charge resistance of 360 degree domain walls reaches a maximum at an intermediate wall thickness, unlike 180 degree domain walls, whose resistance decreases monotonically with wall thickness. The peak amplitude of the spin torque and the optimal thickness of the domain wall to maximize torque for a 360 degree wall are more than twice as large as found for a 180 degree domain wall in the same material, producing a larger domain wall velocity for the 360 degree wall and suggesting unexpected nonlinearities in magnetoelectronic devices incorporating domain wall motion.",0909.3831v1 2010-08-07,Extending Electrical Resistivity Measurements in Micro-scratching of Silicon to Determine Thermal Conductivity of the Metallic Phase Si-II,"Ductile Regime Machining of semiconductors (DRM) offers higher quality of the resulting surfaces. To optimize this process, it is required to understand the thermal kinetics of silicon metallization under pressure. Such understanding is not yet possible since the metallic phases of silicon aren't readily amenable to thermal characterization through direct measurements. This being the case, one has to rely on processing indirect measurement data to deduce refined estimates of the thermal transport properties of pressurized Silicon. A feasible measurement of this sort is the electrical resistivity, since its' variation during indentation and consider is often an indicator of the formation of the metallic silicon phase Si-II under the indenter. This paper, therefore, describes a procedure by which the average thermal conductivity of the metallic phase of silicon, Si-II is extracted from electrical resistivity measurements taken in real time. The procedure is based on teaming a temperature evaluation code to the resistivity measurements thus allowing the extraction of the conductivity as a function of temperature.",1008.1363v1 2013-03-15,Quantum resistance metrology using graphene,"In this paper we review the recent extraordinary progress in the development of a new quantum standard for resistance based on graphene. We discuss the unique properties of this material system relating to resistance metrology and discuss results of the recent highest-ever precision direct comparison of the Hall resistance between graphene and traditional GaAs. We mainly focus our review on graphene expitaxially grown on SiC, a system which so far resulted in the best results. We also brie y discuss progress in the two other graphene material systems, exfoliated graphene and chemical vapour deposition graphene, and make a critical comparison with SiC graphene. Finally we discuss other possible applications of graphene in metrology.",1303.3749v2 2013-07-02,Periodic steps in the resistance vs. temperature characteristics of doped graphite and graphene: evidence of superconductivity?,"We have observed periodically repeated steps in the resistance vs. temperature characteristics of doped Highly Oriented Pyrolytic Graphite and exfoliated doped multi-layer graphene. The observations consist of a series of regularly spaced steps in the resistance vs. temperature curves. The lowest step is observed at a temperature of from 50 to 60 K. Additional steps are observed at multiples of that basic temperature with the highest step temperature being at approximately 270 K. Quenching by a modest applied magnetic field has been observed. The sizes and widths of the observed steps appear to vary and may be related to some sort of aggregation reminiscent of flux vortex pinning. An additional argon ion implantation at reduced energy was done to see if additional defects in the material would yield additional structure. This was observed to yield much sharper resistance steps at temperatures in excess of 200 K in thin exfoliated peels from the implanted surface of the sample and would support the possibility of the steps being related to pancake vortex pinning in a layered superconductor. Unfortunately, as yet, there has been no direct measurement of either the superconducting energy gap nor has a definitive Meissner effect been observed.",1307.0581v1 2014-04-08,Ferromagnetic resonance spin pumping in CoFeB with highly resistive non-magnetic electrodes,"The relative contribution of spin pumping and spin rectification from the ferromagnetic resonance of CoFeB/non-magnetic bilayers was investigated as a function of non-magnetic electrode resistance. Samples with highly resistive electrodes of Ta or Ti exhibit a stronger spin rectification signal, which may result in over-(or under-)estimation of the spin Hall angle of the materials, while those with low resistive electrodes of Pt or Pd show the domination of the inverse spin Hall effect from spin pumping. By comparison with samples of single FM layer and an inverted structure, we provide a proper analysis method to extract spin pumping contribution.",1404.1993v1 2014-10-08,Resistive switching phenomena in TiOx nanoparticle layers for memory applications,"Electrical characteristics of a Co/TiO_x/Co resistive memory device, fabricated by two different methods are reported. In addition to crystalline TiO_2 layers fabricated via conventional atomic layer deposition (ALD), an alternative method has been examined, where TiO_x nanoparticle layers were fabricated via sol-gel. The different devices have shown different hysteresis loops with a unique crossing point for the sol-gel devices. A simple qualitative model is introduced to describe the different current-voltage behaviours by suggesting only one active metal-oxide interface for the ALD devices and two active metal-oxide interfaces for the sol-gel devices. Furthermore, we show that the resistive switching behaviour could be easily tuned by proper interface engineering and that despite having a similar active material, different fabrication methods can lead to dissimilar resistive switching properties.",1410.2019v1 2014-12-19,The Effect of Varying Co layer thickness on the Time-Temperature Characteristics of Co/Sb Semimetal Embedded Magnetic Nanoparticles,"We report the effect of varying cobalt thickness on the temperature-dependent time decay of the electrical resistance of Co/Sb multilayer samples. We find that for a given temperature, a five fold change in the Co thickness produces a 100 fold change in the characteristic decay time of the resistance. We find that the characteristic decay time, as a function of temperature, follows an Arrhenius law. During deposition, the Co evolves single domain magnetic nanoparticles, on the Sb, in either a Volmer-Weber or Stranski-Krastanov growth mode. This metastable state is then encased in 2.5 nm of Sb producing an embedded nanoparticle system. Scanning Tunneling Microscopy (STM) measurements taken before sample aging (annealing at a given temperature for enough time to complete the resistance decay) and after aging show that these nanoparticles undergo morphological transformations during aging. These transformations lead to well defined time dependent decays in both the magnetization and the electrical resistance, making this material an excellent candidate for an electronic time-temperature sensor.",1412.6436v1 2016-07-07,Low temperature Hall effect in bismuth chalcogenides thin films,"Bismuth chalcogenides are the most studied 3D topological insulators. As a rule, at low temperatures thin films of these materials demonstrate positive magnetoresistance due to weak antilocalization. Weak antilocalization should lead to resistivity decrease at low temperatures; in experiments, however, resistivity grows as temperature decreases. From transport measurements for several thin films (with various carrier density, thickness, and carrier mobility), and by using purely phenomenological approach, with no microscopic theory, we show that the low temperature growth of the resistivity is accompanied by growth of the Hall coefficient, in agreement with diffusive electron-electron interaction correction mechanism. Our data reasonably explain the low-temperature resistivity upturn.",1607.02034v2 2017-11-05,Quantification of Dislocation-Precipitate Interactions,"The present research is the first attempt to systematically quantify the dislocation-precipitate interaction in terms of applied shear stress, precipitate resistance, and the required time to reach the critical state of dislocation-precipitate interaction when a dislocation line is about to pass through precipitates. To model the dislocation-precipitate interaction, we adopt a modified three-dimensional dislocation dynamics. Using the present modeling approach, which employs three-dimensional dislocation dynamics simulations, we obtain thousands of data points, accounting for various precipitate resistances, applied shear stresses, and precipitate spacing. The material of reference is Copper (Cu). From the simulations, which quantify the dislocation-precipitate interaction in terms of the applied shear stress, precipitate resistance scale, and dislocation-precipitate interaction time, we found a universal equation. The dislocation-precipitate interaction time versus precipitate resistance and stress, referred to as the ""dislocation-precipitate interaction map,"" determines the ""pass"" or ""no-pass"" state of the interaction. Using this map, we incorporate the dislocation-precipitate interaction time in a two-dimensional multiscale framework which adopts the dislocation dynamics approach at the micro-scale and the finite element method at the macro-scale. We use this framework to model the mechanical behavior of free-standing copper thin films. The results show a dual effect of the dislocation-precipitate interaction time on the hardening level.",1711.01556v1 2018-04-09,Superconductivity from Meissner Effect and Zero Resistivity in a Phenyl Molecule,"Recently, phenyl molecules have been reported to exhibit Meissner effect mainly from magnetization measurements. Realizing zero-resistivity state in these materials seems a challenge due to many practical difficulties but is required to characterize the existence of superconductivity. By choosing potassium-doped tris(2-methylphenyl)bismuthine as an example, we perform temperature-dependent magnetic susceptibility and resistivity measurements at different magnetic fields and pressures. The solid evidence for supporting superconductivity is achieved from the obtained Meissner effect and zero resistivity with the critical temperature ($T_c$) of 3.6 K at atmosphere pressure. Upon compression, we observe the gradual evolution of superconductivity from its initial phase with a parabolic behavior of $T_{c}$ to the second one with almost constant value of $T_{c}$ of 7 K. The 7 K phase seems a common feature for these newly discovered phenyl-based superconductors.",1804.03060v1 2018-09-17,Tetragonal CuMnAs alloy: role of defects,"The antiferromagnetic (AFM) CuMnAs alloy with tetragonal structure is a promising material for the AFM spintronics. The resistivity measurements indicate the presence of defects about whose types and concentrations is more speculated as known. We confirmed vacancies on Mn or Cu sublattices and Mn$_{\rm Cu}$ and Cu$_{\rm Mn}$ antisites as most probable defects in CuMnAs by our new ab initio total energy calculations. We have estimated resistivities of possible defect types as well as resistivities of samples for which the X-ray structural analysis is available. In the latter case we have found that samples with Cu- and Mn-vacancies with low formation energies have also resistivities which agree well with the experiment. Finally, we have also calculated exchange interactions and estimated the N\'eel temperatures by using the Monte Carlo approach. A good agreement with experiment was obtained.",1809.06239v1 2022-02-13,Slow electron-phonon relaxation controls the dynamics of the superconducting resistive transition,"We investigate the temporal and spatial scales of resistance fluctuations (R-fluctuations) at the superconducting resistive transition accessed through voltage fluctuations measurements in thin epitaxial TiN films. This material is characterized by a record slow electron-phonon relaxation, which puts it far beyond the applicability range of the textbook scenario of superconducting fluctuations. The measured Lorentzian spectrum of the R-fluctuations identifies their correlation time, which is nearly constant across the transition region and has no relation to the conventional Ginzburg-Landau time scale. Instead, the correlation time coincides with the energy relaxation time determined by a combination of the electron-phonon relaxation and the diffusion in reservoirs. Our data is quantitatively consistent with the model of spontaneous temperature fluctuations and highlight important caveats in the accepted physical picture of the resistive transition in materials with slow electron-phonon relaxation.",2202.06309v2 2015-07-30,A physics based model of gate tunable metal-graphene contact resistance benchmarked against experimental data,"The metal-graphene contact resistance is a technological bottleneck for the realization of viable graphene based electronics. We report a useful model to find the gate tunable components of this resistance determined by the sequential tunneling of carriers between the 3D-metal and 2D-graphene underneath followed by Klein tunneling to the graphene in the channel. This model quantifies the intrinsic factors that control that resistance, including the effect of unintended chemical doping. Our results agree with experimental results for several metals.",1507.08412v1 2018-07-12,Ultra Low Specific Contact Resistivity in Metal-Graphene Junctions via Atomic Orbital Engineering,"A systematic investigation of graphene edge contacts is provided. Intentionally patterning monolayer graphene at the contact region creates well-defined edge contacts that lead to a 67% enhancement in current injection from a gold contact. Specific contact resistivity is reduced from 1372 {\Omega}m for a device with surface contacts to 456 {\Omega}m when contacts are patterned with holes. Electrostatic doping of the graphene further reduces contact resistivity from 519 {\Omega}m to 45 {\Omega}m, a substantial decrease of 91%. The experimental results are supported and understood via a multi-scale numerical model, based on density-functional-theory calculations and transport simulations. The data is analyzed with regards to the edge perimeter and hole-to-graphene ratio, which provides insights into optimized contact geometries. The current work thus indicates a reliable and reproducible approach for fabricating low resistance contacts in graphene devices. We provide a simple guideline for contact design that can be exploited to guide graphene and 2D material contact engineering.",1807.04772v1 2019-10-18,Resistive contribution in electrical switching experiments with antiferromagnets,"Recent research demonstrated the electrical switching of antiferromagnets via intrinsic spin-orbit torque or the spin Hall effect of an adjacent heavy metal layer. The electrical readout is typically realized by measuring the transverse anisotropic magnetoresistance at planar cross- or star-shaped devices with four or eight arms, respectively. Depending on the material, the current density necessary to switch the magnetic state can be large, often close to the destruction threshold of the device. We demonstrate that the resulting electrical stress changes the film resistivity locally and thereby breaks the fourfold rotational symmetry of the conductor. This symmetry breaking due to film inhomogeneity produces signals, that resemble the anisotropic magnetoresistance and is experimentally seen as a ""saw-tooth""-shaped transverse resistivity. This artifact can persist over many repeats of the switching experiment and is not easily separable from the magnetic contribution. We discuss the origin of the artifact, elucidate the role of the film crystallinity, and propose approaches how to separate the resistive contribution from the magnetic contribution.",1910.08576v1 2020-12-11,Anomalous Hall resistivity and possible topological Hall effect in the EuAl$_4$ antiferromagnet,"We report the observation of anomalous Hall resistivity in single crystals of EuAl$_4$, a centrosymmetric tetragonal compound, which exhibits coexisting antiferromagnetic (AFM) and charge-density-wave (CDW) orders with onset at $T_\mathrm{N} \sim 15.6$ K and $T_\mathrm{CDW} \sim 140$ K, respectively. In the AFM state, when the magnetic field is applied along the $c$-axis direction, EuAl$_4$ undergoes a series of metamagnetic transitions. Within this field range, we observe a clear hump-like anomaly in the Hall resistivity, representing part of the anomalous Hall resistivity. By considering different scenarios, we conclude that such a hump-like feature is most likely a manifestation of the topological Hall effect, normally occurring in noncentrosymmetric materials known to host nontrivial topological spin textures. In view of this, EuAl$_4$ would represent a rare case where the topological Hall effect not only arises in a centrosymmetric structure, but it also coexists with CDW order.",2012.06088v1 2021-05-11,Lattice contraction induced by resistive switching in chromium-doped V2O3: a hallmark of Mott physics,"Since the beginnings of the electronic age, a quest for ever faster and smaller switches has been initiated, since this element is ubiquitous and foundational in any electronic circuit to regulate the flow of current. Mott insulators are promising candidates to meet this need as they undergo extremely fast resistive switching under electric field. However the mechanism of this transition is still under debate. Our spatially-resolved {\mu}-XRD imaging experiments carried out on the prototypal Mott insulator (V0.95Cr0.05)2O3 show that the resistive switching is associated with the creation of a conducting filamentary path consisting in an isostructural compressed phase without any chemical nor symmetry change. This clearly evidences that the resistive switching mechanism is inherited from the bandwidth-controlled Mott transition. This discovery might hence ease the development of a new branch of electronics dubbed Mottronics.",2105.05093v2 2021-06-21,Unique Temperature Distribution and Explicit Efficiency Formula for One-Dimensional Thermoelectric Generators under Constant Seebeck Coefficients,"A thermoelectric generator converts a temperature difference into electrical energy. Its energy conversion efficiency is determined by the steady-state temperature distribution inside the generator. By assuming the thermoelectric material in the generator has a temperature-independent Seebeck coefficient and the generator is one-dimensional, we show that the second-order integro-differential equation describing the inside temperature distribution has a unique solution for any given ratio of external load resistance to the internal resistance. Hence the efficiency is well defined. Furthermore, we show the efficiency has an explicit formula in terms of the temperature-dependent thermal conductivity and electrical resistivity of the thermoelectric material. On the other hand, if we impose an external load resistance value, not the ratio, then the integro-differential equation can have multiple solutions.",2106.10957v1 2022-05-02,Recent advances in inorganic oxides-based resistive random-access memory devices,"Memory has always been a building block element for information technology. Emerging technologies such as artificial intelligence, big data, the internet of things, etc., require a novel kind of memory technology that can be energy efficient and have an exception data retention period. Among several existing memory technologies, resistive random-access memory (RRAM) is an answer to the above question as it is necessary to possess the combination of speed of RAM and nonvolatility, thus proving to be one of the most promising candidates to replace flash memory in next-generation non-volatile RAM applications. This review discusses the existing challenges and technological advancements made with RRAM, including switching mechanism, device structure, endurance, fatigue resistance, data retention period, and mechanism of resistive switching in inorganic oxides material used as a dielectric layer. Finally, a summary and a perspective on future research are presented.",2205.05537v1 2023-01-06,"Spin Transport in Magnetically Ordered Systems: Ferromagnets, Antiferromagnets and Frustrated Systems","In this review, we outline the important results on the resistivity encountered by an electron in magnetically ordered materials. The mechanism of the collision between the electron and the lattice spins is shown. Experiments on the spin resistivity in various magnetic materials as well as theoretical background are recalled. We focus on our works since 15 years using principally Monte Carlo simulations. In these works, we have studied the spin resistivity in various kinds of magnetic systems ranging from ferromagnets and antiferromagnets to frustrated spin systems. It is found that the spin resistivity shows a broad peak at the transition temperature in systems with a second-order phase transition, while it undergoes a discontinuous jump at the transition temperature of a first-order transition. New results on the hexagonal-close-packed (HCP) antiferromagnet are also shown in extended details for the Ising case in both the frustrated and non-frustrated parameter regions.",2301.02689v1 2023-02-27,Analytical expression of negative differential thermal resistance in a macroscopic heterojunction,"Heat flux ($J$) generally increases with temperature difference in a material. A differential coefficient of $J$ against temperature ($T$) is called differential thermal conductance ($k$), and an inverse of $k$ is differential thermal resistance ($r$). Although $k$ and $r$ are generally positive, they can be negative in a macroscopic heterojunction with positive $T$-dependent interfacial thermal resistance (ITR). The negative differential thermal resistance (NDTR) effect is an important effect that can realize thermal transistor, thermal memory, and thermal logic gate. In this paper, we examine analytical expressions of $J$, $k$, $r$, and other related quantities as a function of parameters related to thermal conductivity ($\kappa$) and ITR in a macroscopic heterojunction to precisely describe the NDTR effect.",2302.14065v3 2017-01-18,Role of Thermal Resistance on the Performance of Superconducting Radio Frequency Cavities,"Thermal stability is an important parameter for the operation of the superconducting radio frequency (SRF) cavities used in particle accelerators. The rf power dissipated on the inner surface of the cavities is conducted to the helium bath cooling the outer cavity surface and the equilibrium temperature of the inner surface depends on the thermal resistance. In this manuscript, we present the results of direct measurements of thermal resistance on 1.3 GHz single cell SRF cavities made from high purity large grain and fine grain niobium as well as their rf performance for different treatments applied to outer cavity surface in order to investigate the role of the Kapitza resistance to the overall thermal resistance and to the SRF cavity performance. The results show no significant impact of the thermal resistance to the SRF cavity performance after chemical polishing, mechanical polishing or anodization of the outer cavity surface. Temperature maps taken during the rf test show non-uniform heating of the surface at medium rf fields. Calculations of Q0(Bp) curves using the thermal feedback model show good agreement with experimental data at 2 K and 1.8 K when a pair-braking term is included in the calculation of the BCS surface resistance. These results indicate local intrinsic non-linearities of the surface resistance, rather than purely thermal effects, to be the main cause for the observed field dependence of Q0(Bp).",1701.05097v1 2019-04-13,Quantum Point Contact Parameter Extraction of Carbon-based Resistive Memory using Hybrid Genetic Algorithm,"Resistive switching phenomenon in carbon film is associated with formation and annihilation of low resistance sp2 nanochannels within the amorphous sp3 matrix. The thinnest point of these graphitic nanochannels behaves like quantum wire (QW) and limits current flow. Transport mechanism at these bottlenecks can be described within the framework of quantum point contact (QPC) model. The model applies mesoscopic Landauer formalism and correlates device resistance state with the density of the nanochannels as well as lateral area of its constriction. However, QPC model parameter extraction from macroscopic I-V characteristic is not feasible due to multiple nonlinear and closely coupled parameters, e.g. barrier height ({\Phi}), barrier curvature ({\alpha}) and voltage drop ratio (\b{eta}). In this work, a hybrid genetic algorithm (GA) based parameter extraction flow is proposed and is applied to extract parameters from experimental result of carbon-based resistive memories. In this proposed flow, the number of single subband channels for low resistance state (NLRS) and barrier curvature parameter at high resistance state ({\alpha}HRS) were first derived by exploring boundary conditions at low voltage. The four remaining parameters ({\Phi}HRS, {\Phi}LRS, {\alpha}LRS, and \b{eta}) were then extracted from experimental I-V characteristic by leveraging hybrid GA. Mean absolute percentage error (MAPE) of fitted QPC models is only 3.7% and the extracted parameters are within reasonable range. Hereby, we regard the QPC model as a viable model to describe conduction mechanism of graphitic nanochannels in carbon-based resistive memories.",1904.06542v1 2022-11-16,Unconventional charge-to-spin conversions in graphene/MoTe2 van der Waals heterostructures,"Spin-charge interconversion (SCI) is a central phenomenon to the development of spintronic devices from materials with strong spin-orbit coupling (SOC). In the case of materials with high crystal symmetry, the only allowed SCI processes are those where the spin current, charge current and spin polarization directions are orthogonal to each other. Consequently, standard SCI experiments are designed to maximize the signals arising from the SCI processes with conventional mutually orthogonal geometry. However, in low-symmetry materials, certain non-orthogonal SCI processes are also allowed. Since the standard SCI experiment is limited to charge current flowing only in one direction in the SOC material, certain allowed SCI configurations remain unexplored. In this work, we performed a thorough SCI study in a graphene-based lateral spin valve combined with low-symmetry MoTe$_2$. Due to a very low contact resistance between the two materials, we could detect SCI signals using both a standard configuration, where the charge current is applied along the MoTe$_2$, and a recently introduced (3D-current) configuration, where the charge current flow can be controlled in three directions within the heterostructure. As a result, we observed three different SCI components, one orthogonal and two non-orthogonal, giving new insight into the SCI processes in low-symmetry materials. The large SCI signals obtained at room temperature, along with the versatility of the 3D-current configuration, provide feasibility and flexibility to the design of the next generation of spin-based devices.",2211.09095v1 2001-06-27,Planar Superconductor-Normal-Superconductor Josephson Junctions in MgB2,"Since the discovery of superconductivity in MgB2 considerable progress has been made in determining the physical properties of the material, which are promising for bulk conductors. Tunneling studies show that the material is reasonably isotropic and has a well-developed s-wave energy gap (∆), implying that electronic devices based on MgB2 could operate close to 30K. Although a number of groups have reported the formation of thin films by post-reaction of precursors, heterostructure growth is likely to require considerable technological development, making single-layer device structures of most immediate interest. MgB2 is unlike the cuprate superconductors in that grain boundaries do not form good Josephson junctions, and although a SQUID based on MgB2 nanobridges has been fabricated, the nanobridges themselves do not show junction-like properties. Here we report the successful creation of planar MgB2 junctions by localised ion damage in thin films. The critical current (IC) of these devices is strongly modulated by applied microwave radiation and magnetic field. The product of the critical current and normal state resistance (ICRN) is remarkably high, implying a potential for very high frequency applications.",0106562v1 2008-04-02,Anomalously large measured thermoelectric power factor in Sr$_{1-x}$La$_x$TiO$_3$ thin films due to SrTiO$_3$ substrate reduction,"We report the observation that thermoelectric thin-films of La-doped SrTiO3 grown on SrTiO3 substrates yield anomalously high values of thermopower to give extraordinary values of power factor at 300K. Thin-films of Sr0.98La0.02TiO3, grown via pulsed laser deposition at low temperature and low pressure (450C, 10-7Torr), do not yield similarly high values when grown on other substrates. The thin-film growth induces oxygen reduction in the SrTiO3 crystals, doping the substrate n-type. It is found that the backside resistance of the SrTiO3 substrates is as low (~12ohm/square) as it is on the film-side after film growth.",0804.0443v3 2014-06-13,Superconductivity in single-layer films of FeSe with a transition temperature above 100 K,"Recently, interface has been employed to enhance superconductivity in the single-layer FeSe films grown on SrTiO3(001)(STO) with a possible Tc of ~ 80 K, which is nearly ten times of the Tc of bulk FeSe and is above the Tc record of 56 K for the bulk Fe-based superconductors. This work together with those on superconducting oxides interfaces revives the long-standing idea that electron pairing at a two-dimensional (2D) interface between two different materials is a potential path to high transition temperature (Tc) superconductivity. Subsequent angle-resolved photoemission spectroscopy (ARPES) measurements revealed different electronic structure from those of bulk FeSe with a superconducting-like energy gap closing at around 65K. However, previous ex situ electrical transport measurements could only detect the zero-resistance below ~30 K. Here we report the observation of high Tc superconductivity in the FeSe/STO system. By in situ 4-point probe (4PP) electrical transport measurement that can be conducted at an arbitrary position of the FeSe film on STO, we detected superconductivity above 100 K. Our finding makes FeSe/STO the exciting and ideal research platform for higher Tc superconductivity.",1406.3435v1 2019-05-23,Lattice frustration in spin-orbit Mott insulator Sr3Ir2O7 at high pressure,"The intertwined charge, spin, orbital, and lattice degrees of freedom could endow 5d compounds with exotic properties. Current interest is focused on electromagnetic interactions in these materials, whereas the important role of lattice geometry remains to be fully recognized. For this sake, we investigate pressure-induced phase transitions in the spin-orbit Mott insulator Sr3Ir2O7 with Raman, electrical resistance, and x-ray diffraction measurements. We reveal an interesting magnetic transition coinciding with a structural transition at 14.4 GPa, but without a concurrent insulator-metal transition. The conventional correlation between magnetic and Mott insulating states is thereby absent. The observed softening of the one-magnon mode can be explained by a reduced tetragonal distortion, while the actual magnetic transition is associated with tilting of the IrO6 octahedra. This work highlights the critical role of lattice frustration in determining the high-pressure phases of Sr3Ir2O7. The ability to control electromagnetic properties via manipulating the crystal structure with pressure promises a new way to explore new quantum states in spin-orbit Mott insulators.",1905.09637v1 2019-09-13,Monolayer MoS2 field effect transistor with low Schottky barrier height with ferromagnetic metal contacts,"Two-dimensional MoS2 has emerged as promising material for nanoelectronics and spintronics due to its exotic properties. However, high contact resistance at metal semiconductor MoS2 interface still remains an open issue. Here, we report electronic properties of field effect transistor devices using monolayer MoS2 channels and permalloy (Py) as ferromagnetic (FM) metal contacts. Monolayer MoS2 channels were directly grown on SiO2/Si substrate via chemical vapor deposition technique. The increase in current with back gate voltage shows the tunability of FET characteristics. The Schottky barrier height (SBH) estimated for Py/MoS2 contacts is found to be +28.8 meV (zero-bias), which is the smallest value reported so-far for any direct metal (magnetic or non-magnetic)/monolayer MoS2 contact. With the application of gate voltage (+10 V), SBH shows a drastic reduction down to a value of -6.8 meV. The negative SBH reveals ohmic behavior of Py/MoS2 contacts. Low SBH with controlled ohmic nature of FM contacts is a primary requirement for MoS2 based spintronics and therefore using directly grown MoS2 channels in the present study can pave a path towards high performance devices for large scale applications.",1909.06014v1 2017-03-10,Extremely high conductivity observed in the triple point topological metal MoP,"Weyl and Dirac fermions have created much attention in condensed matter physics and materials science. Recently, several additional distinct types of fermions have been predicted. Here, we report ultra-high electrical conductivity in MoP at low temperature, which has recently been established as a triple point Fermion material. Here we show that the electrical resistivity is 6 n-ohm cm at 2 K with a large mean free path of 11 microns. de Haas-van Alphen oscillations reveal spin splitting of the Fermi surfaces. In contrast to noble metals with similar conductivity and number of carriers, the magnetoresistance in MoP does not saturate up to 9 T at 2 K. Interestingly, the momentum relaxing time of the electrons is found to be more than 15 times larger than the quantum coherence time. This difference between the scattering scales shows that momentum conserving scattering dominates in MoP at low temperatures.",1703.03736v2 2020-09-13,Topologically-Driven Linear Magnetoresistance in Helimagnetic FeP,"The helimagnet FeP is part of a family of binary pnictide materials with the MnP-type structure which share a nonsymmorphic crystal symmetry that preserves generic band structure characteristics through changes in elemental composition. It shows many similarities, including in its magnetic order, to isostructural CrAs and MnP, two compounds that are driven to superconductivity under applied pressure. Here we present a series of high magnetic field experiments on high quality single crystals of FeP, showing that the resistance not only increases without saturation by up to several hundred times its zero field value by 35 T, but that it also exhibits an anomalously linear field dependence over the entire field range when the field is aligned precisely along the crystallographic c-axis. A close comparison of quantum oscillation frequencies to electronic structure calculations links this orientation to a semi-Dirac point in the band structure which disperses linearly in a single direction in the plane perpendicular to field, a symmetry-protected feature of this entire material family. We show that the two striking features of MR-large amplitude and linear field dependence-arise separately in this system, with the latter likely due to a combination of ordered magnetism and topological band structure.",2009.05984v2 2017-04-28,Optimization of the Crystal Growth of the Superconductor CaKFe$_{4}$As$_{4}$ from Solution in the FeAs-CaFe$_{2}$As$_{2}$-KFe$_{2}$As$_{2}$ System,"Measurements of the anisotropic properties of single crystals play a crucial role in probing the physics of new materials. Determining a growth protocol that yields suitable high-quality single crystals can be particularly challenging for multi-component compounds. Here we present a case study of how we refined a procedure to grow single crystals of CaKFe$_{4}$As$_{4}$ from a high temperature, quaternary liquid solution rich in iron and arsenic (""FeAs self-flux""). Temperature dependent resistance and magnetization measurements are emphasized, in addition to the x-ray diffraction, to detect inter-grown CaKFe$_{4}$As$_{4}$, CaFe$_{2}$As$_{2}$ and KFe$_{2}$As$_{2}$ within, what appear to be, single crystals. Guided by the rules of phase equilibria and these data, we adjusted growth parameters to suppress formation of the impurity phases. The resulting optimized procedure yielded phase-pure single crystals of CaKFe$_{4}$As$_{4}$. This optimization process offers insight into the growth of quaternary compounds and a glimpse of the four-component phase diagram in the pseudo-ternary FeAs-CaFe$_{2}$As$_{2}$-KFe$_{2}$As$_{2}$ system.",1704.09025v2 2020-08-15,Low Dimensional Material based Electro-Optic Phase Modulation Performance Analysis,"Electro-optic modulators are utilized ubiquitously ranging from applications in data communication to photonic neural networks. While tremendous progress has been made over the years, efficient phase-shifting modulators are challenged with fundamental tradeoffs, such as voltage-length, index change-losses or energy-bandwidth, and no single solution available checks all boxes. While voltage-driven phase modulators, such as based on lithium niobate, offer low loss and high speed operation, their footprint of 10's of cm-scale is prohibitively large, especially for density-critical applications, for example in photonic neural networks. Ignoring modulators for quantum applications, where loss is critical, here we distinguish between current versus voltage-driven modulators. We focus on the former, since current-based schemes of emerging thin electro-optical materials have shown unity-strong index modulation suitable for heterogeneous integration into foundry waveguides. Here, we provide an in-depth ab-initio analysis of obtainable modulator performance based on heterogeneously integrating low-dimensional materials, i.e. graphene, thin films of indium tin oxide, and transition metal dichalcogenide monolayers into a plurality of optical waveguide designs atop silicon photonics. Using the fundamental modulator tradeoff of energy-bandwidth-product as a design-quality quantifier, we show that a small modal cross section, such as given by plasmonic modes, enables high-performance operation, physically realized by arguments on charge-distribution and low electrical resistance. An in-depth design understanding of phase-modulator performance, beyond doped-junctions in silicon, offers opportunities for micrometer-compact yet energy-bandwidth-ratio constrained modulators with timely opportunities to hardware-accelerate applications beyond data communication towards photonic machine intelligence.",2008.06792v1 2021-03-30,Magnetic Texture in Insulating Single Crystal High Entropy Oxide Spinel Films,"Magnetic insulators are important materials for a range of next generation memory and spintronic applications. Structural constraints in this class of devices generally require a clean heterointerface that allows effective magnetic coupling between the insulating layer and the conducting layer. However, there are relatively few examples of magnetic insulators which can be synthesized with surface qualities that would allow these smooth interfaces and precisely tuned interfacial magnetic exchange coupling which might be applicable at room temperature. In this work, we demonstrate an example of how the configurational complexity in the magnetic insulator layer can be used to realize these properties. The entropy-assisted synthesis is used to create single crystal (Mg0.2Ni0.2Fe0.2Co0.2Cu0.2)Fe2O4 films on substrates spanning a range of strain states. These films show smooth surfaces, high resistivity, and strong magnetic responses at room temperature. Local and global magnetic measurements further demonstrate how strain can be used to manipulate magnetic texture and anisotropy. These findings provide insight into how precise magnetic responses can be designed using compositionally complex materials that may find application in next generation magnetic devices.",2103.16722v1 2022-08-03,"Reactive Laser Synthesis of Ultra-high-temperature Ceramics HfC, ZrC, TiC, HfN, ZrN, and TiN for Additive Manufacturing","Ultra-high-temperature ceramics (UHTCs) are optimal structural materials for applications that require extreme temperature resilience, resistance to chemically aggressive environments, wear, and mechanical stress. Processing UHTCs with laser-based additive manufacturing (AM) has not been fully realized due to a variety of obstacles. In this work, selective laser reaction sintering (SLRS) techniques were investigated for the production of near net-shape UHTC ceramics such as HfC, ZrC, TiC, HfN, ZrN, and TiN. Group IV transition metal and metal oxide precursor materials were chemically converted and reaction-bonded into layers of UHTCs using single-step selective laser processing in CH4 or NH3 gas that might be compatible with prevailing powder bed fusion techniques. Conversion of either metals (Hf, Zr and Ti) or metal oxides (HfO2, ZrO2, and TiO2) particles was first investigated to examine reaction mechanisms and volume changes associated with SLRS of single-component precursor systems. SLRS processing of metal or metal oxide alone produced near stoichiometric UHTC phases with yields up to 100 wt% total for carbides and nitrides. However, for single component precursors, gas-solid reactivity induced volumetric changes resulted in residual stresses and cracking in the product layer. To mitigate conversion-induced stresses, composite metal/metal oxide precursors were employed to compensate for the volume changes of either the metal (which expands during conversion) or the metal oxide precursor (which contracts).",2208.02041v2 2023-04-24,Absolute radiation tolerance of amorphous alumina coatings at room temperature,"In this study structural and mechanical properties of a 1 um thick Al2O3 coating, deposited on 316L stainless steel by Pulsed Laser Deposition (PLD), subjected to high energy ion irradiation were assessed. Mechanical properties of pristine and ion-modified specimens were investigated using the nanoindentation technique. A comprehensive characterization combining Transmission Electron Microscopy and Grazing-Incidence X-ray Diffraction provided deep insight into the structure of the tested material at the nano- and micro- scale. Variation in the local atomic ordering of the irradiated zone at different doses was investigated using a reduced distribution function analysis obtained from electron diffraction data. Findings from nanoindentation measurements revealed a slight reduction in hardness of all irradiated layers. At the same time TEM examination indicated that the irradiated layer remained amorphous over the whole dpa range. No evidence of crystallization, void formation or element segregation was observed up to the highest implanted dose. Reported mechanical and structural findings were critically compared with each other pointing to the conclusion that under given irradiation conditions, over the whole range of doses used, alumina coatings exhibit excellent radiation resistance. Obtained data strongly suggest that investigated material may be considered as a promising candidate for next-generation nuclear reactors, especially LFR-type, where high corrosion protection is one of the highest prerogatives to be met.",2304.11973v1 2023-06-01,"Nonlinear characteristics of Ti, Nb, and NbN superconducting resonators for parametric amplifiers","Superconducting resonators and parametric amplifiers are important components in scientific systems such as kinetic inductance detector arrays, frequency-domain multiplexers for other superconducting bolometers, spin-ensemble based memories, and circuit quantum electrodynamics demonstrators. In this paper, we report microwave measurements of superconducting Ti, Nb, and NbN resonators and their use as parametric amplifiers. These half-wave resonators were fabricated under near identical sputtering and lithographic conditions to ensure a like-for-like comparison of material properties. We report a wide range of properties and behaviours in terms of transition temperatures, resistivities, rate-limiting nonlinear response times, nonlinear dissipation, signs of the nonlinear inductances and their dependences on temperature and resonance harmonic. We have successfully operated Nb and NbN resonators as high gain parametric amplifiers, achieving greater than $20\,\mathrm{dB}$ of power amplification. We have shown that for a half-wave resonator, amplification can be realised not only in the fundamental resonance but also in the higher harmonic resonances. Further, for materials with high transition temperatures, e.g. Nb and NbN, amplification can be achieved at $\sim4\,\mathrm{K}$, i.e. a temperature maintained by a pulse tube cooler. Finally, in materials systems that have very fast response times, e.g. NbN, we have found that a cross-harmonic type of amplification can be achieved by placing pump tone in a different resonant mode as the signal and the idler. This wide range of observations will have important implications on the design and application of superconducting parametric amplifiers.",2306.00685v2 2023-07-17,MBE growth of axion insulator candidate EuIn2As2,"The synthesis of thin films of magnetic topological materials is necessary to achieve novel quantized Hall effects and electrodynamic responses. EuIn2As2 is a recently predicted topological axion insulator that has an antiferromagnetic ground state and an inverted band structure, but that has only been synthesized and studied as a single crystal. We report on the synthesis of c-axis oriented EuIn2As2 films on sapphire substrates by molecular beam epitaxy. By carefully tuning the substrate temperature during growth, we stabilize the Zintl phase of EuIn2As2 expected to be topologically non-trivial. The magnetic properties of these films reproduce those seen in single crystals, but their resistivity is enhanced when grown at lower temperatures. We additionally find that the magnetoresistance of EuIn2As2 is negative even up to fields as high as 31T. while it is highly anisotropic at low fields, it becomes nearly isotropic at high magnetic fields above 5T. Overall, the transport characteristics of EuIn2As2 appear similar to those of chalcogenide topological insulators, motivating the development of devices to gate tune the Fermi energy and reveal topological features in quantum transport.",2307.08831v2 2023-12-20,Singular Hall response from a correlated ferromagnetic flat nodal-line semimetal,"Topological quantum phases have been largely understood in weakly correlated systems, which have identified various quantum phenomena such as spin Hall effect, protected transport of helical fermions, and topological superconductivity. Robust ferromagnetic order in correlated topological materials particularly attracts attention, as it can provide a versatile platform for novel quantum devices. Here, we report singular Hall response arising from a unique band structure of flat topological nodal lines in combination with electron correlation in an itinerant, van der Waals ferromagnetic semimetal, Fe3GaTe2, with a high Curie temperature of Tc=360 K. High anomalous Hall conductivity violating the conventional scaling, resistivity upturn at low temperature, and a large Sommerfeld coefficient are observed in Fe3GaTe2, which implies heavy fermion features in this ferromagnetic topological material. Our circular dichroism in angle-resolved photoemission spectroscopy and theoretical calculations support the original electronic features in the material. Thus, low-dimensional Fe3GaTe2 with electronic correlation, topology, and room-temperature ferromagnetic order appears to be a promising candidate for robust quantum devices.",2312.12889v1 2024-02-28,Multifunctional composite magnet for practical transverse thermoelectrics,"Permanent magnets are used in various products and essential for human society. If omnipresent permanent magnets could directly convert heat into electricity, they would lead to innovative energy harvesting and thermal management technologies. However, achieving such ""multifunctionality"" has been difficult because of the poor thermoelectric performance of conventional magnets. Here, we develop a multifunctional composite magnet that enables giant transverse thermoelectric conversion. The proposed composite material, comprising alternately and obliquely stacked SmCo$_5$/Bi$_{0.2}$Sb$_{1.8}$Te$_3$ multilayers, exhibits large remanent magnetization and coercivity as well as an excellent figure of merit of 0.32 for transverse thermoelectric conversion around room temperature. While having versatile transverse geometry and high mechanical durability, the thermopile module based on these composite magnets generates 204 mW at a temperature difference of 152 K owing to extremely low interfacial electrical and thermal resistances. The corresponding power density per heat transfer area of 56.7 mW/cm$^2$ is not only record-high among all the transverse thermoelectric modules but also comparable to those of commercial longitudinal thermoelectric modules based on the Seebeck effect. The novel functional material enables the integration of thermoelectric conversion capabilities wherever permanent magnets are currently used.",2402.18019v1 1996-06-05,Hall Resistivity in Ferromagnetic Manganese-Oxide Compounds,"Temperature-dependence and magnetic field-dependence of the Hall effect and the magnetic property in manganese-oxide thin films are studied. The spontaneous magnetization and the Hall resistivity are obtained for a various of magnetic fields over all the temperature. It is shown that the Hall resistivity in small magnetic field is to exhibit maximum near the Curie point, and strong magnetic field moves the position of the Hall resistivity peak to much high temperature and suppresses the peak value. The change of the Hall resistance in strong magnetic field may be larger than that of the diagonal ones. The abnormal Hall resistivity in the ferromagnetic manganese-oxide thin-films is attributed to the spin-correlation fluctuation scattering.",9606030v1 2002-06-04,Free flux flow resistivity in strongly overdoped high-T_c cuprate; purely viscous motion of the vortices in semiclassical d-wave superconductor,"We report the free flux flow (FFF) resistivity associated with a purely viscous motion of the vortices in moderately clean d-wave superconductor Bi:2201 in the strongly overdoped regime (T_c=16K) for a wide range of the magnetic field in the vortex state. The FFF resistivity is obtained by measuring the microwave surface impedance at different microwave frequencies. It is found that the FFF resistivity is remarkably different from that of conventional s-wave superconductors. At low fields (H<0.2H_c2) the FFF resistivity increases linearly with H with a coefficient which is far larger than that found in conventional s-wave superconductors. At higher fields, the FFF resistivity increases in proportion to \sqrt H up to H_c2. Based on these results, the energy dissipation mechanism associated with the viscous vortex motion in ""semiclassical"" d-wave superconductors with gap nodes is discussed. Two possible scenarios are put forth for these field dependence; the enhancement of the quasiparticle relaxation rate and the reduction of the number of the quasiparticles participating the energy dissipation in d-wave vortex state.",0206031v1 2003-06-14,Radiation induced zero-resistance states in GaAs/AlGaAs heterostructures: Voltage-current characteristics and intensity dependence at the resistance minima,"High mobility two-dimensional electron systems exhibit vanishing resistance over broad magnetic field intervals upon excitation with microwaves, with a characteristic reduction of the resistance with increasing radiation intensity at the resistance minima. Here, we report experimental results examining the voltage - current characteristics, and the resistance at the minima vs. the microwave power. The findings indicate that a non-linear V-I curve in the absence of microwave excitation becomes linearized under irradiation, unlike expectations, and they suggest a similarity between the roles of the radiation intensity and the inverse temperature.",0306388v2 2007-05-12,Effects of electromagnetic waves on the electrical properties of contacts between grains,"A DC electrical current is injected through a chain of metallic beads. The electrical resistances of each bead-bead contacts are measured. At low current, the distribution of these resistances is large and log-normal. At high enough current, the resistance distribution becomes sharp and Gaussian due to the creation of microweldings between some beads. The action of nearby electromagnetic waves (sparks) on the electrical conductivity of the chain is also studied. The spark effect is to lower the resistance values of the more resistive contacts, the best conductive ones remaining unaffected by the spark production. The spark is able to induce through the chain a current enough to create microweldings between some beads. This explains why the electrical resistance of a granular medium is so sensitive to the electromagnetic waves produced in its vicinity.",0705.1775v2 2009-12-10,Dichotomy in the $T$-linear resistivity in hole-doped cuprates,"From analysis of the in-plane resistivity $\rho_{ab}(T)$ of La$_{2-x}$Sr$_x$CuO$_4$, we show that normal state transport in overdoped cuprates can be delineated into two regimes in which the electrical resistivity varies approximately linearly with temperature. In the low temperature limit, the $T$-linear resistivity extends over a very wide doping range, in marked contrast to expectations from conventional quantum critical scenarios. The coefficient of this $T$-linear resistivity scales with the superconducting transition temperature $T_c$, implying that the interaction causing this anomalous scattering is also associated with the superconducting pairing mechanism. At high temperatures, the coefficient of the $T$-linear resistivity is essentially doping independent beyond a critical doping $p_{\rm crit}$ = 0.19 at which the ratio of the two coefficients is maximal. Taking our cue from earlier thermodynamic and photoemission measurements, we conclude that the opening of the normal state pseudogap at $p_{\rm crit}$ is driven by the loss of coherence of anti-nodal quasiparticles at low temperatures.",0912.2001v1 2010-05-25,Resistive Magnetohydrodynamic Simulations of Relativistic Magnetic Reconnection,"Resistive relativistic magnetohydrodynamic (RRMHD) simulations are applied to investigate the system evolution of relativistic magnetic reconnection. A time-split Harten--Lan--van Leer method is employed. Under a localized resistivity, the system exhibits a fast reconnection jet with an Alfv\'{e}nic Lorentz factor inside a narrow Petschek-type exhaust. Various shock structures are resolved in and around the plasmoid such as the post-plasmoid vertical shocks and the ""diamond-chain"" structure due to multiple shock reflections. Under a uniform resistivity, Sweet--Parker-type reconnection slowly evolves. Under a current-dependent resistivity, plasmoids are repeatedly formed in an elongated current sheet. It is concluded that the resistivity model is of critical importance for RRMHD modeling of relativistic magnetic reconnection.",1005.4485v2 2013-12-18,Magneto-transport characteristics of a 2D electron system driven to negative magneto-conductivity by microwave photoexcitation,"Negative diagonal magneto-conductivity/resistivity is a spectacular- and thought provoking- property of driven, far-from-equilibrium, low dimensional electronic systems. The physical response of this exotic electronic state is not yet fully understood since it is rarely encountered in experiment. The microwave-radiation-induced zero-resistance state in the high mobility GaAs/AlGaAs 2D electron system is believed to be an example where negative magneto-conductivity/resistivity is responsible for the observed phenomena. Here, we examine the magneto-transport characteristics of this negative conductivity/resistivity state in the microwave photo-excited two-dimensional electron system (2DES) through a numerical solution of the associated boundary value problem. The results suggest, surprisingly, that a bare negative diagonal conductivity/resistivity state in the 2DES under photo-excitation should yield a positive diagonal resistance with a concomitant sign reversal in the Hall voltage.",1312.5026v1 2014-12-19,Nano-artifact metrics based on random collapse of resist,"Artifact metrics is an information security technology that uses the intrinsic characteristics of a physical object for authentication and clone resistance. Here, we demonstrate nano-artifact metrics based on silicon nanostructures formed via an array of resist pillars that randomly collapse when exposed to electron-beam lithography. The proposed technique uses conventional and scalable lithography processes, and because of the random collapse of resist, the resultant structure has extremely fine-scale morphology with a minimum dimension below 10 nm, which is less than the resolution of current lithography capabilities. By evaluating false match, false non-match and clone-resistance rates, we clarify that the nanostructured patterns based on resist collapse satisfy the requirements for high-performance security applications.",1412.6271v1 2015-07-15,ERK/p38 MAPK inhibition reduces radio-resistance to pulsed proton beam in breast cancer stem cells cells,"Recent studies have identified highly tumorigenic cells with stem cell-like characteristics in human cancers, termed cancer stem cells (CSCs). CSCs are resistant to conventional radiotherapy and chemotherapy owing to their high DNA repair ability and oncogene overexpression. However, the mechanisms regulating CSC radio-resistance, particularly proton beam resistance, remain unclear. We isolated CSCs from the breast cancer cell lines MCF-7 and MDA-MB-231, which expressed the characteristic breast CSC membrane protein markers CD44+/CD24-/low, and irradiated the CSCs with pulsed proton beams. We confirmed that CSCs are resistant to pulsed proton beams and showed that treatment with p38 and ERK inhibitors reduced CSC radioresistance. Based on these results, BCSC radio-resistance can be reduced during proton beam therapy by co-treatment with ERK1/2 or p38 inhibitors, representing a novel approach for breast cancer therapy.",1509.02377v1 2017-06-23,Investigating prescriptions for artificial resistivity in smoothed particle magnetohydrodynamics,"In numerical simulations, artificial terms are applied to the evolution equations for stability. To prove their validity, these terms are thoroughly tested in test problems where the results are well known. However, they are seldom tested in production-quality simulations at high resolution where they interact with a plethora of physical and numerical algorithms. We test three artificial resistivities in both the Orszag-Tang vortex and in a star formation simulation. From the Orszag-Tang vortex, the Price et. al. (2017) artificial resistivity is the least dissipative thus captures the density and magnetic features; in the star formation algorithm, each artificial resistivity algorithm interacts differently with the sink particle to produce various results, including gas bubbles, dense discs, and migrating sink particles. The star formation simulations suggest that it is important to rely upon physical resistivity rather than artificial resistivity for convergence.",1706.07721v1 2019-07-05,Impurity scattering induced carrier transport in twisted bilayer graphene,"We theoretically calculate the impurity-scattering induced resistivity of twisted bilayer graphene at low twist angles where the graphene Fermi velocity is strongly suppressed. We consider, as a function of carrier density, twist angle, and temperature, both long-ranged Coulomb scattering and short-ranged defect scattering within a Boltzmann theory relaxation time approach. For experimentally relevant disorder, impurity scattering contributes a resistivity comparable to (much larger than) the phonon scattering contribution at high (low) temperatures. Decreasing twist angle leads to larger resistivity, and in general, the resistivity increases (decreases) with increasing temperature (carrier density). Inclusion of the van Hove singularity in the theory leads to a strong increase in the resistivity at higher densities, where the chemical potential is close to a van Hove singularity, leading to an apparent density-dependent plateau type structure in the resistivity, which has been observed in recent transport experiments. We also show that the Matthissen's rule is strongly violated in twisted bilayer graphene at low twist angles.",1907.02856v3 2021-01-28,Contagion-Preserving Network Sparsifiers: Exploring Epidemic Edge Importance Utilizing Effective Resistance,"Network epidemiology has become a vital tool in understanding the effects of high-degree vertices, geographic and demographic communities, and other inhomogeneities in social structure on the spread of disease. However, many networks derived from modern datasets are quite dense, such as mobility networks where each location has links to a large number of potential destinations. One way to reduce the computational effort of simulating epidemics on these networks is sparsification, where we select a representative subset of edges based on some measure of their importance. Recently an approach was proposed using an algorithm based on the effective resistance of the edges. We explore how effective resistance is correlated with the probability that an edge transmits disease in the SI model. We find that in some cases these two notions of edge importance are well correlated, making effective resistance a computationally efficient proxy for the importance of an edge to epidemic spread. In other cases, the correlation is weaker, and we discuss situations in which effective resistance is not a good proxy for epidemic importance.",2101.11818v1 2023-02-22,Drugs Resistance Analysis from Scarce Health Records via Multi-task Graph Representation,"Clinicians prescribe antibiotics by looking at the patient's health record with an experienced eye. However, the therapy might be rendered futile if the patient has drug resistance. Determining drug resistance requires time-consuming laboratory-level testing while applying clinicians' heuristics in an automated way is difficult due to the categorical or binary medical events that constitute health records. In this paper, we propose a novel framework for rapid clinical intervention by viewing health records as graphs whose nodes are mapped from medical events and edges as correspondence between events in given a time window. A novel graph-based model is then proposed to extract informative features and yield automated drug resistance analysis from those high-dimensional and scarce graphs. The proposed method integrates multi-task learning into a common feature extracting graph encoder for simultaneous analyses of multiple drugs as well as stabilizing learning. On a massive dataset comprising over 110,000 patients with urinary tract infections, we verify the proposed method is capable of attaining superior performance on the drug resistance prediction problem. Furthermore, automated drug recommendations resemblant to laboratory-level testing can also be made based on the model resistance analysis.",2302.11231v2 2023-11-03,Resistive Diffusion in Magnetized ICF Implosions: Reduced Magnetic Stabilization of the Richtmyer Meshkov Instability,"Resistive diffusion is typically regarded to be negligible in magnetized ICF experiments, with magnetic flux effectively compressed during the implosion. In this work the Richtmyer Meshkov instability at the ice-ablator interface is taken as an example for investigating resistive effects. For a high temperature (approximately 100eV) interface with magnetic field applied perpendicular to shock propagation, perturbation growth is suppressed by magnetic tension. However, for lower temperature interfaces the resistive diffusion prevents substantial magnetic field twisting at small scales. ICF implosion simulations are then used to assess magnetic diffusivity at different interfaces; the ice-ablator interface is found to be too resistive for the magnetic fields to enhance stability. For Rayleigh-Taylor growth at the hot-spot edge, on the other hand, resistivity is estimated to only be a secondary effect, as seen in previous simulation studies.",2311.01645v2 2024-03-14,Role of many phonon modes on the high-temperature linear-in-$T$ electronic resistivity,"We theoretically consider the possibility that phonons may be playing a role in the observed linear-in-$T$ resistivity in cuprates by focusing on the obvious question: How can phonon scattering be consistent with a linear-in-$T$ resistivity with a constant slope given that cuprates have many phonon modes with different energies and electron-phonon couplings (e.g. 21 phonon modes for LSCO)? We show using an arbitrarily large number of independent phonon modes that, within a model Boltzmann transport theory, the emergent high-$T$ linear-in-$T$ resistivity manifests an approximately constant slope independent of the number of phonon modes except in some fine-tuned narrow temperature regimes. We also comment on the quantitative magnitude of the linear-in-$T$ resistivity in cuprates pointing out the constraints on the effective electron-phonon coupling necessary to produce the observed resistivity.",2403.09890v1 2017-02-16,Anomalous Nonlocal Resistance and Spin-charge Conversion Mechanisms in Two-Dimensional Metals,"We uncover two anomalous features in the nonlocal transport behavior of two-dimensional metallic materials with spin-orbit coupling. Firstly, the nonlocal resistance can have negative values and oscillate with distance, even in the absence of a magnetic field. Secondly, the oscillations of the nonlocal resistance under an applied in-plane magnetic field (Hanle effect) can be asymmetric under field reversal. Both features are produced by direct magnetoelectric coupling, which is possible in materials with broken inversion symmetry but was not included in previous spin diffusion theories of nonlocal transport. These effects can be used to identify the relative contributions of different spin-charge conversion mechanisms. They should be observable in adatom-functionalized graphene, and may provide the reason for discrepancies in recent nonlocal transport experiments on graphene.",1702.04955v3 2018-06-23,Crack growth resistance in metallic alloys: the role of isotropic versus kinematic hardening,"The sensitivity of crack growth resistance to the choice of isotropic or kinematic hardening is investigated. Monotonic mode I crack advance under small scale yielding conditions is modelled via a cohesive zone formulation endowed with a traction-separation law. R-curves are computed for materials that exhibit linear or power law hardening. Kinematic hardening leads to an enhanced crack growth resistance relative to isotropic hardening. Moreover, kinematic hardening requires greater crack extension to achieve the steady state. These differences are traced to the non-proportional loading of material elements near the crack tip as the crack advances. The sensitivity of the R-curve to the cohesive zone properties and to the level of material strain hardening is explored for both isotropic and kinematic hardening.",1806.08986v1 2020-01-08,Novel hypostasis of old materials in oxide electronics: metal oxides for resistive random access memory applications,"Transition-metal oxide films, demonstrating the effects of both threshold and nonvolatile memory resistive switching, have been recently proposed as candidate materials for storage-class memory. In this work we describe some experimental results on threshold switching in a number of various transition metal (V, Ti, Fe, Nb, Mo, W, Hf, Zr, Mn, Y, and Ta) oxide films obtained by anodic oxidation. Then, the results concerning the effects of bistable resistive switching in MOM and MOS structures on the basis of such oxides as V2O5, Nb2O5, and NiO are presented. It is shown that sandwich structures on the basis of the Au/V2O5/SiO2/Si, Nb/Nb2O5/Au, and Pt/NiO/Pt can be used as memory elements for ReRAM applications. Finally, model approximations are developed in order to describe theoretically the effect of nonvolatile unipolar switching in Pt NiO-Pt structures.",2001.03026v1 2022-04-28,Ultralow Electron-Surface Scattering in Nanoscale Metals Leveraging Fermi Surface Anisotropy,"Increasing resistivity of metal wires with reducing nanoscale dimensions is a major performance bottleneck of semiconductor computing technologies. We show that metals with suitably anisotropic Fermi velocity distributions can strongly suppress electron scattering by surfaces and outperform isotropic conductors such as copper in nanoscale wires. We derive a corresponding descriptor for the resistivity scaling of anisotropic conductors, screen thousands of metals using first-principles calculations of this descriptor and identify the most promising materials for nanoscale interconnects. Previously-proposed layered conductors such as MAX phases and delafossites show promise in thin films, but not in narrow wires due to increased scattering from side walls. We find that certain intermetallics (notably CoSn) and borides (such as YCo$_3$B$_2$) with one-dimensionally anisotropic Fermi velocities are most promising for narrow wires. Combined with first-principles electron-phonon scattering predictions, we show that the proposed materials exhibit 2-3x lower resistivity than copper at 5 nm wire dimensions.",2204.13458v1 2022-07-20,Optimal Structures for Failure Resistance Under Impact,"The complex physics and numerous failure modes of structural impact creates challenges when designing for impact resistance. While simple geometries of layered material are conventional, advances in 3D printing and additive manufacturing techniques have now made tailored geometries or integrated multi-material structures achievable. Here, we apply gradient-based topology optimization to the design of such structures. We start by constructing a variational model of an elastic-plastic material enriched with gradient phase-field damage, and present a novel method to efficiently compute its transient dynamic time evolution. We consider a finite element discretization with explicit updates for the displacements. The damage field is solved through an augmented Lagrangian formulation, splitting the operator coupling between the nonlinearity and non-locality. Sensitivities over this trajectory are computed through the adjoint method, resulting in an adjoint problem which we solve in a similar manner to the forward dynamics. We demonstrate this formulation by studying the optimal design of 2D solid-void structures undergoing blast loading. Then, we explore the trade-offs between strength and toughness in the design of a spall-resistant structure composed of two materials of differing properties undergoing dynamic impact.",2207.09678v1 1998-05-11,"Two-dimensional arrays of low capacitance tunnel junctions: general properties, phase transitions and Hall effect","We describe transport properties of two-dimensional arrays of low capacitance tunnel junctions, such as the current voltage characteristic and its dependence on external magnetic field and temperature. We discuss several experiments in which the small capacitance of the junctions plays an important role. In arrays where the junctions have a relatively large charging energy, (i.e. when they have a low capacitance) and a high normal state resistance, the low bias resistance increases with decreasing temperature and eventually at very low temperature the array becomes insulating even though the electrodes in the array are superconducting. This transition to the insulating state can be described by thermal activation. In an intermediate region where the junction resistance is of the order of the quantum resistance and the charging energy is of the order of the Josephson coupling energy, the arrays can be tuned between a superconducting and an insulating state with a magnetic field. We describe measurements of this magnetic-field-tuned superconductor insulator transition, and we show that the resistance data can be scaled over several orders of magnitude. Four arrays follow the same universal function. At the transition the transverse (Hall) resistance is found to be very small in comparison with the longitudinal resistance. However, for magnetic field values larger than the critical value.we observe a substantial Hall resistance. The Hall resistance of these arrays oscillates with the applied magnetic field. features in the magnetic field dependence of the Hall resistance can qualitatively be correlated to features in the derivative of the longitudinal resistance, similar to what is found in the quantum Hall effect.",9805121v1 2020-07-03,First-principles study of electronic transport and structural properties of Cu$_{12}$Sb$_4$S$_{13}$ in its high-temperature phase,"We present an ab initio study of the structural and electronic transport properties of tetrahedrite, Cu$_{12}$Sb$_4$S$_{13}$, in its high-temperature phase. We show how this complex compound can be seen as the outcome of an ordered arrangement of S-vacancies in a semiconducting fematinite-like structure (Cu3SbS4). Our calculations confirm that the S-vacancies are the natural doping mechanism in this thermoelectric compound and reveal a similar local chemical environment around crystallographically inequivalent Cu atoms, shedding light on the debate on XPS measurements in this compound. To access the electrical transport properties as a function of temperature we use the Kubo-Greenwood formula applied to snapshots of first-principles molecular dynamics simulations. This approach is essential to effectively account for the interaction between electrons and lattice vibrations in such a complex crystal structure where a strong anharmonicity plays a key role in stabilising the high-temperature phase. Our results show that the Seebeck coeffcient is in good agreement with experiments and the phonon-limited electrical resistivity displays a temperature trend that compares well with a wide range of experimental data. The predicted lower bound for the resistivity turns out to be remarkably low for a pristine mineral in the Cu-Sb-S system but not too far from the lowest experimental data reported in literature. The Lorenz number turns out to be substantially lower than what expected from the free-electron value in the Wiedemann-Franz law, thus providing an accurate way to estimate the electronic and lattice contributions to the thermal conductivity in experiments, of great significance in this very low thermal conductivity crystalline material.",2007.01809v2 2015-03-25,Anisotropy of Thermal Conductivity of Free-Standing Reduced Graphene Oxide Films Annealed at High Temperature,"We investigated thermal conductivity of free-standing reduced graphene oxide films subjected to a high-temperature treatment of up to 1000 C. It was found that the high-temperature annealing dramatically increased the in-plane thermal conductivity, K, of the films from 3 W/mK to 61 W/mK at room temperature. The cross-plane thermal conductivity, Kc, revealed an interesting opposite trend of decreasing to a very small value of 0.09 W/mK in the reduced graphene oxide films annealed at 1000 C. The obtained films demonstrated an exceptionally strong anisotropy of the thermal conductivity, K/Kc ~ 675, which is substantially larger even than in the high-quality graphite. The electrical resistivity of the annealed films reduced to 1 - 19 Ohms/sq. The observed modifications of the in-plane and cross-plane thermal conductivity components resulting in an unusual K/Kc anisotropy were explained theoretically. The theoretical analysis suggests that K can reach as high as ~500 W/mK with the increase in the sp2 domain size and further reduction of the oxygen content. The strongly anisotropic heat conduction properties of these films can be useful for applications in thermal management.",1503.07239v1 2017-03-07,Thermodynamic Stabilization of Precipitates through Interface Segregation: Chemical Effects,"Precipitation hardening, which relies on a high density of intermetallic precipitates, is a commonly utilized technique for strengthening structural alloys. Structural alloys are commonly strengthened through a high density of small size intermetallic precipitates. At high temperatures, however, the precipitates coarsen to reduce the excess energy of the interface, resulting in a significant reduction in the strengthening provided by the precipitates. In certain ternary alloys, the secondary solute segregates to the interface and results in the formation of a high density of nanosize precipitates that provide enhanced strength and are resistant to coarsening. To understand the chemical effects involved, and to identify such systems, we develop a thermodynamic model using the framework of the regular nanocrystalline solution model. For various global compositions, temperatures and thermodynamic parameters, equilibrium configuration of Mg-Sn-Zn alloy is evaluated by minimizing the Gibbs free energy function with respect to the region-specific (bulk solid-solution, interface and precipitate) concentrations and sizes. The results show that Mg$_2$Sn precipitates can be stabilized to nanoscale sizes through Zn segregation to Mg/Mg$_2$Sn interface, and the precipitates can be stabilized against coarsening at high-temperatures by providing a larger Zn concentration in the system. Together with the inclusion of elastic strain energy effects and the input of computationally informed interface thermodynamic parameters in the future, the model is expected to provide a more realistic prediction of segregation and precipitate stabilization in ternary alloys of structural importance.",1703.02621v2 2020-09-29,High open-circuit voltage in transition metal dichalcogenide solar cells,"The conversion efficiency of ultra-thin solar cells based on layered materials has been limited by their open-circuit voltage, which is typically pinned to a value under 0.6 V. Here we report an open-circuit voltage of 1.02 V in a 120 nm-thick vertically stacked homojunction fabricated with substitutionally doped MoS2. This high open-circuit voltage is consistent with the band alignment in the MoS2 homojunction, which is more favourable than in widely-used TMDC heterostructures. It is also attributed to the high performance of the substitutionally doped MoS2, in particular the p-type material doped with Nb, which is demonstrated by the observation of electroluminescence from tunnelling graphene/BN/MoS2 structures in spite of the indirect nature of bulk MoS2. We find that illuminating the TMDC/metal contacts decreases the measured open-circuit voltage in MoS2 van der Waals homojunctions because they are photoactive, which points to the need of developing low-resistance, ohmic contacts to doped MoS2 in order to achieve high efficiency in practical devices. The high open-circuit voltage demonstrated here confirms the potential of layered transition-metal dichalcogenides for the development of highly efficient, ultra-thin solar cells.",2009.13911v1 2019-11-25,Natural-mixing guided design of refractory high-entropy alloys with as-cast tensile ductility,"Multi-principal-element metallic alloys have created a growing interest that is unprecedented in metallurgical history, in exploring the property limits of metals and the governing physical mechanisms. Refractory high-entropy alloys (RHEAs) have drawn particular attention due to their (i) high melting points and excellent softening-resistance, which are the two key requirements for high-temperature applications; and (ii) compositional space, which is immense even after considering cost and recyclability restrictions. However, RHEAs also exhibit intrinsic brittleness and oxidation-susceptibility, which remain as significant challenges for their processing and application. Here, utilizing natural-mixing characteristics amongst refractory elements, we designed a Ti38V15Nb23Hf24 RHEA that exhibits >20% tensile ductility already at the as-cast state, and physicochemical stability at high-temperatures. Exploring the underlying deformation mechanisms across multiple length-scales, we observe that a rare beta prime precipitation strengthening mechanism governs its intriguing mechanical response. These results also reveal the effectiveness of natural-mixing tendencies in expediting HEA discovery.",1911.10975v1 2021-12-23,Record High Tc Element Superconductivity Achieved In Titanium,"It is challenging to search for high Tc superconductivity (SC) in transition metal elements wherein d electrons are usually not favored by conventional BCS theory. Here we report discovery of surprising SC up to 310 GPa with Tc above 20 K in wide pressure range from 108 GPa to 240 GPa in titanium. The maximum Tc^onset above 26 K and zero resistance Tc^zero of 21 K are record high values hitherto achieved among element superconductors. The Hc2(0) is estimated to be about 32 Tesla with coherence length 32 angstrom. The results show strong s-d transfer and d-band dominance, indicating correlation driven contributions to high Tc SC in dense titanium. This finding is in sharp contrast to the theoretical predications based on pristine electron-phonon coupling scenario. The study opens a fresh promising avenue for rational design and discovery of high Tc superconductors among simple materials via pressure tuned unconventional mechanism.",2112.12396v3 2022-01-12,Emergence of superconducting dome in insulating ZrNx films via nitrogen manipulation,"Reproducing the electronic phase diagram of strongly correlated high-transition-temperature (high-Tc) superconductors in materials other than Cu-, Fe-, and Ni-based compounds has been a challenging task. Only very recently, a few material systems have partially achieved this goal by band engineering. In this work, we combine film growth, charge transport, magnetometry, Terahertz Spectroscopy, Raman scattering, and Scanning Transmission Electron Microscopy to investigate superconductivity and the normal state of ZrNx, which reveals a phase diagram that bears extraordinary similarities to those of high-Tc superconductors. Remarkably, even though superconductivity of ZrNx can be characterized within the Bardeen-Cooper-Schrieffer paradigm and its normal state can be understood within the Fermi liquid framework, by tunning the N chemical concentration, we observe the evolution of a superconducting dome in the close vicinity of a strongly insulating state and a normal state resistivity mimics its counterpart of the high-Tc superconductors.",2201.04340v2 2023-06-22,Scalable Electrodeposition of Eutectic Indium Gallium from an Acetonitrile-Based Electrolyte for Integrated Stretchable Electronics,"For the advancement of highly-integrated stretchable electronics, the development of scalable sub-micrometer conductor patterning is required. Eutectic gallium indium EGaIn is an attractive conductor for stretchable electronics, as its liquid metallic character grants it high electrical conductivity upon deformation. However, its high surface energy precludes patterning it with (sub)-micron resolution. Herein, we overcome this limitation by reporting for the first time the electrodeposition of EGaIn. We use a non-aqueous acetonitrile-based electrolyte that exhibits high electrochemical stability and chemical orthogonality. The electrodeposited material led to low-resistance lines that remained stable upon (repeated) stretching to a 100 percent strain. Because electrodeposition benefits from the resolution of mature nanofabrication methods used to pattern the base metal, the proposed bottom-up approach achieved a record-high density integration of EGaIn regular lines of 300 nm half-pitch on an elastomer substrate by plating on a gold seed layer pre-patterned by nanoimprinting. Moreover, vertical integration was enabled by filling high aspect ratio vias. This capability was conceptualized by the fabrication of an omnidirectionally stretchable 3D electronic circuit, and demonstrates a soft-electronic analogue of the stablished damascene process used to fabricate microchip interconnects. Overall, this work proposes a simple route to address the challenge of metallization in highly integrated (3D) stretchable electronics.",2306.12781v2 2020-05-28,High-temperature and Abrasion Resistant Selective Solar Absorber under Ambient Environment,"Selective solar absorbers (SSAs) with high performance are the key to concentrated solar power systems. Optical metamaterials are emerging as a promising strategy to enhance selective photon absorption, however, the high-temperature resistance (>500C) remains as one of the main challenges for their practical applications. Here, a multilayered metamaterial system (Al2O3/W/SiO2/W) based on metal-insulator-metal (MIM) resonance effect has been demonstrated with high solar absorptance over 92%, low thermal emittance loss below 6%, and significant high-temperature resistance: it has been proved that the optical performance remains 93.6% after 1-hour thermal annealing under ambient environment up to 500C, and 94.1% after 96-hour thermal cycle test at 400C, which is also confirmed by the microscopic morphology characterization. The spectral selectivity of fabricated SSAs is angular independent and polarization insensitive. Outdoor tests demonstrate that a peak temperature rise (193.5C) can be achieved with unconcentrated solar irradiance and surface abrasion resistance test yields that SSAs have a robust resistance to abrasion attack for engineering applications.",2005.14305v1 2015-11-22,On materials destruction criteria,"In terms of nonlinear material fracture mechanics, the real (discrete)-structure material fracture model has been developed. The model rests on the demonstration of the fact that crack resistance $K_{1c}=2\sigma \sqrt l$ and fracture toughness are $G_{1c}=J_{1c}=2\sigma l$ obtained on the basis of energy conservation law and derived without linear material fracture mechanics assumptions can be respectively taken as force and energy criteria for non-linear fracture mechanics. It is shown that $G_{1c}=K_{1c}^2/E$ is the energy criterion of linear fracture mechanics of material and it is sufficiently less than $G_{1c} = J_{1c}=2\sigma l$.",1511.07037v1 2021-01-31,"Origin of high hardness and optoelectronic and thermo-physical properties of boron-rich compounds B6X (X = S, Se): a comprehensive study via DFT approach","In the present study, the structural and hitherto uninvestigated mechanical (elastic stiffness constants, machinability index, Cauchy pressure, anisotropy indices, brittleness/ductility, Poissons ratio), electronic, optical, and thermodynamic properties of novel boron-rich compounds B6X (X = S, Se) have been explored using density functional theory. The estimated structural lattice parameters were consistent with the prior report. The mechanical and dynamical stability of these compounds have been established theoretically. The materials are brittle in nature and elastically anisotropic. The value of fracture toughness, KIC for the B6S and B6Se are ~ 2.07 MPam0.5, evaluating the resistance to limit the crack propagation inside the materials. Both B6S and B6Se compounds possess high hardness values in the range 31-35 GPa, and have the potential to be prominent members of the class of hard compounds. Strong covalent bonding and sharp peak at low energy below the Fermi level confirmed by partial density of states (PDOS) resulted in the high hardness. The profile of band structure, as well as DOS, assesses the indirect semiconducting nature of the titled compounds. The comparatively high value of Debye temperature ({\Theta}D), minimum thermal conductivity (Kmin), lattice thermal conductivity (kph), low thermal expansion coefficient, and low density suggest that both boron-rich chalcogenides might be used as thermal management materials. Large absorption capacities in the mid ultraviolet region (3.2-15 eV) of the studied materials and low reflectivity (~16 %) are significantly noted. Such favorable features give promise to the compounds under investigation to be used in UV surface-disinfection devices as well as medical sterilizer equipment applications. Excellent correlations are found among all the studied physical properties of these compounds.",2102.00446v1 2022-10-09,High-performance non-Fermi-liquid metallic thermoelectric materials,"Searching for high-performance thermoelectric (TE) materials in the paradigm of narrow-bandgap semiconductors has lasted for nearly 70 years and is obviously hampered by a bottleneck of research now. Here we report on the discovery of a few metallic compounds, TiFexCu2x-1Sb and TiFe1.33Sb, showing the thermopower exceeding many TE semiconductors and the dimensionless figure of merits comparable with the state-of-the-art TE materials. A quasi-linear temperature (T) dependence of electrical resistivity in 2 K - 700 K and the logarithmic T-dependent electronic specific heat at low temperature are also observed to coexist with the high thermopower, highlighting the strong intercoupling of the non-Fermi-liquid (NFL) quantum critical behavior of electrons with TE transports. Electronic structure analysis reveals the existence of fluctuating Fe-eg-related local magnetic moments, Fe-Fe antiferromagnetic (AFM) interaction at the nearest 4c-4d sites, and two-fold degenerate eg orbitals antiferromagnetically coupled with the dual-type itinerant electrons close to the Fermi level, all of which infer to a competition between the AFM ordering and Kondo-like spin compensation as well as a parallel two-channel Kondo effect. These effects are both strongly meditated by the structural disorder due to the random filling of Fe/Cu at the equivalent 4c/4d sites of the Heusler crystal lattice. The magnetic susceptibility deviates from ideal antiferromagnetism but can be fitted well by x(T) = 1/({\theta} + BT{\alpha}), seemingly being consistent with the quantum critical scenario of strong local correlation as discussed before. Our work not only breaks the dilemma that the promising TE materials should be heavily-doped semiconductors, but also demonstrates the correlation among high TE performance, NFL quantum criticality, and magnetic fluctuation, which opens up new directions for future research.",2210.04201v1 1997-01-06,The role of intermediate layers in the c-axis conductivity of layered superconductors,"A simplified model of c axis transport in the high T_c superconductors is presented. Expressions are found for the c axis optical conductivity, the d.c. resistivity, and the c axis penetration depth. Within the framework of this model, the pseudogap in the optical conductivity arises naturally as a result of the layered band structure of the high T_c materials. We discuss the occurence of the pseudogap in terms of three parameters: a band gap Delta_{ps}, a temperature dependent scattering rate Gamma(T), and the strength of the interlayer coupling t_{perp}. We are also able to find analytic expressions for the d.c. conductivity and the low temperature penetration depth in terms of these three parameters. This work is an attempt to present a simple, unified picture of c axis properties in the high T_c cuprates.",9701029v2 1999-06-01,Current dependence of grain boundary magnetoresistance in La_0.67Ca_0.33MnO_3 films,"We prepared epitaxial ferromagnetic manganite films on bicrystal substrates by pulsed laser ablation. Their low- and high-field magnetoresistance (MR) was measured as a function of magnetic field, temperature and current. At low temperatures hysteretic changes in resistivity up to 70% due to switching of magnetic domains at the coercitive field are observed. The strongly non-ohmic behavior of the current-voltage leads to a complete suppression of the MR effect at high bias currents with the identical current dependence at low and high magnetic fields. We discuss the data in view of tunneling and mesoscale magnetic transport models and propose an explicit dependence of the spin polarization on the applied current in the grain boundary region.",9906007v1 2001-04-02,Antiferromagnetic vortex state in a high-temperature superconductor,"There is strong evidence that magnetic interactions play a crucial role in the mechanism driving high-temperature superconductivity in cuprate superconductors. To investigate this further we have done neutron scattering experiments on the simplest high-temperature superconductor La(2-x)Sr(x)CuO(4) (LSCO) in an applied magnetic field. Below the superconducting transition temperature (Tc), the field penetrates the material via an array of normal state inclusions or vortices while phase coherent superconductivity characterized by zero resistance is suppressed to the lower field-dependent irreversibility temperature. The measurements described here were performed on underdoped LSCO (x=0.10), which develops static incommensurate order below Tc in zero field. Our results show that application of a magnetic field enhances this response without changing the onset temperature. For H=5T the field-induced signal saturates to three times the zero-field signal and phase coherent superconductivity is established within the antiferromagnetic phase.",0104026v1 2004-02-13,High performance n-doped carbon nanotube field-effect transistors,"We describe a robust technique for the fabrication of high performance vertically scaled n-doped field-effect transistors from large band gap carbon nanotubes. These devices have a tunable threshold voltage in the technologically relevant range (-1.3V < V_th < 0.5V) and can carry up to 5-6 muA of current in the on-state. We achieve such performance by exposure to potassium (K) vapor and device annealing in high vacuum. The treatment has a two-fold effect to: (i) controllably shift V_th toward negative gate biases via bulk doping of the nanotube (up to about 0.6e/nm), and (ii) increase the on-current by 1-2 orders of magnitude. This current enhancement is achieved by lowering external device resistance due to more intimate contact between K metal and doped nanotube channel in addition to potential reduction of the Schottky barrier height at the contact.",0402350v1 2005-04-03,Dependence of Giant Tunnel Magnetoresistance of Sputtered CoFeB/MgO/CoFeB Magnetic Tunnel Junctions on MgO Barrier Thickness and Annealing Temperatur,"We investigated the dependence of giant tunnel magnetoresistance (TMR) on the thickness of an MgO barrier and on the annealing temperature of sputtered CoFeB/MgO/CoFeB magnetic tunnel junctions deposited on SiO2/Si wafers. The resistance-area product exponentially increases with MgO thickness, indicating that the quality of MgO barriers is high in the investigated thickness range of 1.15-2.4 nm. High-resolution transmission electron microscope images show that annealing at 375 C results in the formation of crystalline CoFeB/MgO/CoFeB structures, even though CoFeB electrodes are amorphous in the as-sputtered state. The TMR ratio increases with annealing temperature and is as high as 260% at room temperature and 403% at 5 K.",0504051v1 2006-05-09,Subgap conductivity in SIN-junctions of high barrier transparency,"We investigate the current-voltage characteristics of high-transparency superconductor-insulator-normal metal (SIN) junctions with the specific tunnel resistance below 30 kOhm per square micron. The junctions were fabricated from different superconducting and normal conducting materials, including Nb, Al, AuPd and Cu. The subgap leakage currents were found to be appreciably larger than those given by the standard tunnelling model. We explain our results using the model of two-electron tunnelling in the coherent diffusive transport regime. We demonstrate that even in the high-transparency SIN-junctions, a noticeable reduction of the subgap current can be achieved by splitting a junction into several submicron sub-junctions. These structures can be used as nonlinear low-noise shunts in Rapid-Single-Flux-Quantum (RSFQ) circuitry for controlling Josephson qubits.",0605237v2 2002-09-09,Long-term damage induced by hadrons in silicon detectors for uses at the LHC-accelerator and in space missions,"In the present paper, the phenomenological model developed by the authors in previous papers has been used to evaluate the degradation induced by hadron irradiation at the future accelerator facilities or by cosmic protons in high resistivity silicon detectors. The damage has been analysed at the microscopic (defects production and their evolution toward equilibrium) and at the macroscopic level (changes in the leakage current of the p-n junction). The rates of production of primary defects, as well as their evolution toward equilibrium have been evaluated considering explicitly the type of the projectile particle and its energy. Vacancy-interstitial annihilation, interstitial migration to sink, complex (VP, VO, CiOi, CiCs) and divacancy formation are taken into account for different initial silicon material. The influence of these defects on the leakage detector current has been calculated in the frame of the Schokley-Read-Hall model.",0209086v2 2006-11-20,Correlation between radiation processes in silicon and long-time degradation of detectors for high energy physics experiments,"In this contribution, the correlation between fundamental interaction processes induced by radiation in silicon and observable effects which limit the use of silicon detectors in high energy physics experiments is investigated in the frame of a phenomenological model which includes: generation of primary defects at irradiation starting from elementary interactions in silicon; kinetics of defects, effects at the p-n junction detector level. The effects due to irradiating particles (pions, protons, neutrons), to their flux, to the anisotropy of the threshold energy in silicon, to the impurity concentrations and resistivity of the starting material are investigated as time, fluence and temperature dependences of detector characteristics. The expected degradation of the electrical parameters of detectors in the complex hadron background fields at LHC & SLHC are predicted.",0611185v1 2008-07-11,Electronic liquid crystal state in the high-temperature superconductor YBCO(6.45),"Electronic phases with symmetry properties matching those of conventional liquid crystals have recently been discovered in transport experiments on semiconductor heterostructures and metal oxides at milli-Kelvin temperatures. We report the spontaneous onset of a onedimensional, incommensurate modulation of the spin system in the high-temperature superconductor YBa2Cu3O6.45 upon cooling below ~150 K, while static magnetic order is absent above 2 K. The evolution of this modulation with temperature and doping parallels that of the in-plane anisotropy of the resistivity, indicating an electronic nematic phase that is stable over a wide temperature range. The results suggest that soft spin fluctuations are a microscopic route towards electronic liquid crystals, and nematic order can coexist with high-temperature superconductivity in underdoped cuprates.",0807.1861v1 2009-08-20,"Scaling relation of the anomalous Hall effect in (Ga,Mn)As","We present magnetotransport studies performed on an extended set of (Ga,Mn)As samples at 4.2 K with longitudinal conductivities sigma_{xx} ranging from the low- to the high-conductivity regime. The anomalous Hall conductivity sigma_{xy}^(AH) is extracted from the measured longitudinal and Hall resistivities. A transition from sigma_{xy}^(AH)=20 Omega^{-1}cm^{-1} due to the Berry phase effect in the high-conductivity regime to a scaling relation sigma_{xy}^(AH) proportional to sigma_{xx}^{1.6} for low-conductivity samples is observed. This scaling relation is consistent with a recently developed unified theory of the anomalous Hall effect in the framework of the Keldysh formalism. It turns out to be independent of crystallographic orientation, growth conditions, Mn concentration, and strain, and can therefore be considered universal for low-conductivity (Ga,Mn)As. The relation plays a crucial role when deriving values of the hole concentration from magnetotransport measurements in low-conductivity (Ga,Mn)As. In addition, the hole diffusion constants for the high-conductivity samples are determined from the measured longitudinal conductivities.",0908.2935v1 2009-11-11,Temperature dependent nucleation and annihilation of individual magnetic vortices,"We studied the temperature dependence of the magnetization reversal in individual submicron permalloy disks with micro-Hall and bend-resistance magnetometry. The nucleation field exhibits a nonmonotonic dependence with positive and negative slopes at low and high temperatures, respectively, while the annihilation field monotonically decreases with increasing temperature, but with distinctly different slopes at low and high temperatures. Our analysis suggests that at low temperatures vortex nucleation and annihilation proceeds via thermal activation over an energy barrier, while at high temperatures they are governed by a temperature dependence of the saturation magnetization.",0911.2267v1 2009-12-08,Correlating the nanostructure and electronic properties of InAs nanowires,"The electronic properties and nanostructure of InAs nanowires are correlated by creating multiple field effect transistors (FETs) on nanowires grown to have low and high defect density segments. 4.2 K carrier mobilities are ~4X larger in the nominally defect-free segments of the wire. We also find that dark field optical intensity is correlated with the mobility, suggesting a simple route for selecting wires with a low defect density. At low temperatures, FETs fabricated on high defect density segments of InAs nanowires showed transport properties consistent with single electron charging, even on devices with low resistance ohmic contacts. The charging energies obtained suggest quantum dot formation at defects in the wires. These results reinforce the importance of controlling the defect density in order to produce high quality electrical and optical devices using InAs nanowires.",0912.1511v2 2012-05-30,A Path to Higher Q0 with Large Grain Niobium Cavities,"The improvement of the quality factor Q0 of superconducting radio-frequency (SRF) cavities at medium accelerating gradients (20-25 MV/m) is important in order to reduce the cryogenic losses in continuous wave (CW) accelerators used for a variety of applications. In recent years, SRF cavities fabricated from ingot niobium have become a viable alternative to standard high-purity fine-grain Nb for the fabrication of high-performing SRF cavities with the possibility of significant cost reduction. Recent studies demonstrated the improvement of Q0 at medium field in cavities heat treated at 800-1200 {\deg}C without subsequent chemical etching [ ]. To further explore this treatment procedure, a new induction furnace with an all-niobium hot-zone was commissioned [ ]. A single-cell 1.5 GHz cavity fabricated from ingot material from CBMM, Brazil, with RRR 200, was heat treated in the new furnace in the temperature range 800-1400 {\deg}C for several hours. Residual resistance value of 1 - 5 n\Omega have been consistently achieved on this cavity Q0-values as high as 4.6\times1010 at 90 mT peak surface magnetic field at 2 K. Q0 values of about ~2\times1011 have been measured at 1.5 K.",1205.6736v1 2013-01-23,Superconductivity of interface layer at contact between normal metal and high temperature superconductor,"In this research, it is shown that there are the necessary physical conditions to originate the returning superconductivity in the thin interface layer at the contact between the normal metal and the high temperature superconductor (N-S contact). The influences by the temperature T, magnetic field H and direct current I on the electrical resistance RG of the thin interface layer G in the multilayered system N-G-S, where N can be one the normal metal layers of Argentum (Ag), Indium (In), Gallium-Indium (Ga-50%In), G is the thin interface layer, S is the high temperature superconductor (HTS) layer of YBa2Cu3O7-x, are researched experimentally.",1301.5542v2 2015-03-23,Gate-tunable high mobility remote-doped InSb/In_{1-x}Al_{x}Sb quantum well heterostructures,"Gate-tunable high-mobility InSb/In_{1-x}Al_{x}Sb quantum wells (QWs) grown on GaAs substrates are reported. The QW two-dimensional electron gas (2DEG) channel mobility in excess of 200,000 cm^{2}/Vs is measured at T=1.8K. In asymmetrically remote-doped samples with an HfO_{2} gate dielectric formed by atomic layer deposition, parallel conduction is eliminated and complete 2DEG channel depletion is reached with minimal hysteresis in gate bias response of the 2DEG electron density. The integer quantum Hall effect with Landau level filling factor down to 1 is observed. A high-transparency non-alloyed Ohmic contact to the 2DEG with contact resistance below 1{\Omega} \cdot mm is achieved at 1.8K.",1503.06710v1 2015-09-10,Crystal Structure of 200 K-Superconducting Phase of Sulfur Hydride System,"This article reports the experimentally clarified crystal structure of a recently discovered sulfur hydride in high temperature superconducting phase which has the highest critical temperature Tc over 200 K which has been ever reported. For understanding the mechanism of the high superconductivity, the information of its crystal structure is very essential. Herein we have carried out the simultaneous measurements electrical resistance and synchrotron x-ray diffraction under high pressure, and clearly revealed that the hydrogen sulfide, H2S, decomposes to H3S and its crystal structure has body-centered cubic symmetry in the superconducting phase.",1509.03156v1 2015-09-13,High-Mobility Holes in Dual-Gated WSe$_2$ Field-Effect Transistors,"We demonstrate dual-gated $p$-type field-effect transistors (FETs) based on few-layer tungsten diselenide (WSe$_2$) using high work-function platinum source/drain contacts, and a hexagonal boron nitride top-gate dielectric. A device topology with contacts underneath the WSe$_2$ results in $p$-FETs with $I_{ON}$/$I_{OFF}$ ratios exceeding 10$^7$, and contacts that remain Ohmic down to cryogenic temperatures. The output characteristics show current saturation and gate tunable negative differential resistance. The devices show intrinsic hole mobilities around 140 cm$^2$/Vs at room temperature, and approaching 4,000 cm$^2$/Vs at 2 K. Temperature-dependent transport measurements show a metal-insulator transition, with an insulating phase at low densities, and a metallic phase at high densities. The mobility shows a strong temperature dependence consistent with phonon scattering, and saturates at low temperatures, possibly limited by Coulomb scattering, or defects.",1509.03896v1 2016-08-02,High Current Density and Low Thermal Conductivity of Atomically Thin Semimetallic WTe2,"Two-dimensional (2D) semimetals beyond graphene have been relatively unexplored in the atomically-thin limit. Here we introduce a facile growth mechanism for semimetallic WTe2 crystals, then fabricate few-layer test structures while carefully avoiding degradation from exposure to air. Low-field electrical measurements of 80 nm to 2 um long devices allow us to separate intrinsic and contact resistance, revealing metallic response in the thinnest encapsulated and stable WTe2 devices studied to date (3 to 20 layers thick). High-field electrical measurements and electro-thermal modeling demonstrate that ultra-thin WTe2 can carry remarkably high current density (approaching 50 MA/cm2, higher than most common interconnect metals) despite a very low thermal conductivity (of the order ~3 W/m/K). These results suggest several pathways for air-stable technological viability of this layered semimetal.",1608.00988v1 2016-10-25,Pressure-induced superconductivity in the giant Rashba system BiTeI,"At ambient pressure, BiTeI is the first material found to exhibit a giant Rashba splitting of the bulk electronic bands. At low pressures, BiTeI undergoes a transition from trivial insulator to topological insulator. At still higher pressures, two structural transitions are known to occur. We have carried out a series of electrical resistivity and AC magnetic susceptibility measurements on BiTeI at pressure up to ~40 GPa in an effort to characterize the properties of the high-pressure phases. A previous calculation found that the high-pressure orthorhombic P4/nmm structure BiTeI is a metal. We find that this structure is superconducting with Tc values as high as 6 K. AC magnetic susceptibility measurements support the bulk nature of the superconductivity. Using electronic structure and phonon calculations, we compute Tc and find that our data is consistent with phonon-mediated superconductivity.",1610.08038v1 2016-11-27,Strained GaN Quantum-Well FETs on Single Crystal Bulk AlN Substrates,"We report the first realization of molecular beam epitaxy grown strained GaN quantum well field-effect transistors on single-crystal bulk AlN substrates. The fabricated double heterostructure FETs exhibit a two- dimensional electron gas (2DEG) density in excess of 2x10^13/cm2. Ohmic contacts to the 2DEG channel were formed by n+ GaN MBE regrowth process, with a contact resistance of 0.13 Ohm-mm. Raman spectroscopy using the quantum well as an optical marker reveals the strain in the quantum well, and strain relaxation in the regrown GaN contacts. A 65-nm-long rectangular-gate device showed a record high DC drain current drive of 2.0 A/mm and peak extrinsic transconductance of 250 mS/mm. Small-signal RF performance of the device achieved current gain cutoff frequency fT~120 GHz. The DC and RF performance demonstrate that bulk AlN substrates offer an attractive alternative platform for strained quantum well nitride transistors for future high-voltage and high-power microwave applications.",1611.08914v1 2017-09-19,Design parameter space for a High Pressure Optimized Dense Plasma Focus operating with Deuterium,"The potential of the Dense Plasma Focus (DPF) for industrial applications in many fields is well recognized, although yet to be realized in practice. Particularly attractive is the possibility of its use as inexpensive industrial source of nuclear reactions for diverse high value applications such as fast pulsed neutron radiography of hydrogenous materials, non-intrusive neutron interrogation of concealed organic contraband and rapid production of short lived radioisotopes for medical diagnostics and therapy. Recently, it has been suggested that it may be possible to operate the DPF efficiently in a High-Pressure-Optimized (HPO) mode. This paper explores the design parameter space for such HPO-DPF based on the revised Resistive Gratton-Vargas (RGV) model with a view to identify a practicable set of system parameters and their scaling. The current waveform predicted by the revised RGV model for the chosen set of parameters is fitted to the Lee model to estimate the likely neutron yield.",1709.06243v1 2017-12-09,Extremely large magnetoresistance and high-density Dirac-like fermions in ZrB2,"We report the detailed study on transport properties of ZrB2 single crystal, a predicted topological nodal-line semimetal. ZrB2 exhibits extremely large magnetoresistance as well as field-induced resistivity upturn and plateau. These behaviors can be well understood by the two-band model with the perfect electron - hole compensation and high carrier mobilities. More importantly, the electrons with small effective masses and nontrivial Berry phase have significantly high density when compared to those in known topological semimetals. It strongly suggests that ZrB2 hosts Dirac-like nodal-line fermions.",1712.03362v1 2018-11-01,Ultra-thin low frequency perfect sound absorber with high ratio of active area,"A concept of ultra-thin low frequency perfect sound absorber is proposed and demonstrated experimentally. To minimize non-linear effects, an high ratio of active area to total area is used to avoid large localized amplitudes. The absorber consists of three elements: a mass supported by a very flexible membrane, a cavity and a resistive layer. The resonance frequency of the sound absorber can be easily adjusted just by changing the mass or thickness of the cavity. A very large ratio between wavelength and material thickness is measured for a manufactured perfect absorber (ratio = 201) . It is shown that this high sub-wavelength ratio is associated with narrowband effects and that the increase in the sub-wavelength ratio is limited by the damping in the system.",1811.00897v1 2019-06-28,High pO2 Floating Zone Crystal Growth of the Perovskite Nickelate PrNiO3,"Single crystals of PrNiO3 were grown under an oxygen pressure of 295 bar using a unique high-pressure optical-image floating zone furnace. The crystals, with volume in excess of 1 mm3, were characterized structurally using single crystal and powder X-ray diffraction. Resistivity, specific heat, and magnetic susceptibility were measured, all of which evidenced an abrupt, first order metal-insulator transition (MIT) at ~130 K, in agreement with previous literature reports on polycrystalline specimens. Temperature-dependent single crystal diffraction was performed to investigate changes through the MIT. Our study demonstrates the opportunity space for high fugacity, reactive environments for single crystal growth specifically of perovskite nickelates but more generally to correlated electron oxides.",1907.00078v1 2020-02-17,Characterization of High-Purity Germanium (Ge) Crystals for Developing Novel Ge Detectors,"High-purity germanium (HPGe) crystals are required to be well-characterized before being fabricated into Ge detectors. The characterization of HPGe crystals is often performed with the Hall Effect system, which measures the carrier concentration, the Hall mobility, and the electrical resistivity. The reported values have a strong dependence on the size of the ohmic contacts and the geometry of the samples used in conducting the Hall Effect measurements. We conduct a systematic study using four samples cut from the same location in a HPGe crystal made into different sized ohmic contacts or different geometries to study the variation of the measured parameters from the Hall Effect system. The results are compared to the C-V measurements provided by the Ge detector made from the same crystal. We report the systematic errors involved with the Hall Effect system and find a reliable technique that minimizes the systematic error to be only a few percent from the Hall Effect measurements.",2002.07706v2 2016-03-13,A sub-1-volt analog metal oxide memristive-based synaptic device for energy-efficient spike-based computing systems,"Nanoscale metal oxide memristors have potential in the development of brain-inspired computing systems that are scalable and efficient1-3. In such systems, memristors represent the native electronic analogues of the biological synapses. However, the characteristics of the existing memristors do not fully support the key requirements of synaptic connections: high density, adjustable weight, and low energy operation. Here we show a bilayer memristor that is forming-free, low-voltage (~|0.8V|), energy-efficient (full On/Off switching at ~2pJ), and reliable. Furthermore, pulse measurements reveal the analog nature of the memristive device, that is it can be directly programmed to intermediate resistance states. Leveraging this finding, we demonstrate spike-timing-dependent plasticity (STDP), a spike-based Hebbian learning rule4. In those experiments, the memristor exhibits a marked change in the normalized synaptic strength (>30 times) when the pre- and post-synaptic neural spikes overlap. This demonstration is an important step towards the physical construction of high density and high connectivity neural networks.",1603.03979v1 2017-07-24,Probing local lattice distortion in medium- and high-entropy alloys,"The atomic-level tunability that results from alloying multiple transition metals with d electrons in concentrated solid solution alloys (CSAs), including high-entropy alloys (HEAs), has produced remarkable properties for advanced energy applications, in particular, damage resistance in high-radiation environments. The key to understanding CSAs radiation performance is quantitatively characterizing their complex local physical and chemical environments. In this study, the local structure of a FeCoNiCrPd HEA is quantitatively analyzed with X-ray total scattering and extended X-ray absorption fine structure methods. Compared to FeCoNiCr and FeCoNiCrMn, FeCoNiCrPd with a quasi-random alloy structure has a strong local lattice distortion, which effectively pins radiation-induced defects. Distinct from a relaxation behavior in FeCoNiCr and FeCoNiCrMn, ion irradiation further enhanced the local lattice distortion in FeCoNiCrPd due to a preference for forming Pd-Pd atomic pairs.",1707.07745v1 2019-12-02,Probing intraband excitations in ZrTe$_5$: a high-pressure infrared and transport study,"Zirconium pentatetelluride, ZrTe5, shows remarkable sensitivity to hydrostatic pressure. In this work we address the high-pressure transport and optical properties of this compound, on samples grown by flux and charge vapor transport. The high-pressure resistivity is measured up to 2 GPa, and the infrared transmission up to 9 GPa. The dc conductivity anisotropy is determined using a microstructured sample. Together, the transport and optical measurements allow us to discern band parameters with and without the hydrostatic pressure, in particular the Fermi level, and the effective mass in the less conducting, out-of-plane direction. The results are interpreted within a simple two-band model characterized by a Dirac-like, linear in-plane band dispersion, and a parabolic out-of-plane dispersion.",1912.00942v2 2019-12-23,Change of electronic properties on transition from high-entropy to Ni-rich (TiZrNbCu)(1-x)Ni(x) alloys,"We present results of comprehensive study of electronic properties of (TiZrNbCu)(1-x)Ni(x) metallic glasses performed in broad composition range x encompassing both, high entropy (HE) range, and conventional Ni-base alloy concentration range, x >= 0.35. The electronic structure studied by photoemission spectroscopy and low temperature specific heat (LTSH) reveal a split-band structure of density of states inside valence band with d-electrons of Ti, Zr, Nb and also Ni present at Fermi level N(E_F), whereas LTSH and magnetoresistivity results show that variation of N(E_F) with x changes in Ni-base regime. The variation of superconducting transition temperatures with x closely follows that of N(E_F). The electrical resistivities of all alloys are high and decrease with increasing temperature over most of explored temperature range, and their temperature dependence seems dominated by weak localization effects over a broad temperature range (10-300 K). The preliminary study of Hall effect shows positive Hall coefficient that decreases rapidly in Ni-base alloys.",1912.11133v1 2012-03-27,Graphene-Graphite Quilts for Thermal Management of High-Power GaN Transistors,"Self-heating is a severe problem for high-power GaN electronic and optoelectronic devices. Various thermal management solutions, e.g. flip-chip bonding or composite substrates have been attempted. However, temperature rise still limits applications of the nitride-based technology. Here we demonstrate that thermal management of GaN transistors can be substantially improved via introduction of the alternative heat-escaping channels implemented with few-layer graphene - an excellent heat conductor. We have transferred few-layer graphene to AlGaN/GaN heterostructure field-effect transistors on SiC substrates to form the ""graphene-graphite quilts"" - lateral heat spreaders, which remove heat from the channel regions. Using the micro-Raman spectroscopy for in-situ monitoring we have shown that temperature can be lowered by as much as ~ 20oC in such devices operating at ~13-W/mm power density. The simulations suggest that the efficiency of the ""graphene quilts"" can be made even higher in GaN devices on thermally resistive sapphire substrates and in the designs with the closely located heat sinks. Our results open a novel application niche for few-layer graphene in high-power electronics.",1203.6099v1 2018-12-06,Technologies for Future Vertex and Tracking Detectors at CLIC,"CLIC is a proposed linear $e^{+}e^{-}$ collider with center-of-mass energies of up to $3\,\textrm{TeV}$. Its main objectives are precise top quark and Higgs boson measurements, as well as searches for Beyond Standard Model physics. To meet the physics goals, the vertex and tracking detectors require not only a spatial resolution of a few micrometers and a very low material budget, but also timing capabilities with a precision of a few nanoseconds to allow suppression of beam-induced backgrounds. Different technologies using hybrid silicon detectors are explored for the vertex detectors, such as dedicated readout ASICs, small-pitch active edge sensors as well as capacitively coupled High-Voltage CMOS sensors. Monolithic sensors are considered as an option for the tracking detector, and a prototype using a CMOS process with a high-resistivity epitaxial layer is being designed. Different designs using a silicon-on-insulator process are under investigation for both vertex and tracking detector. All prototypes are evaluated in laboratory and beam tests, and newly developed simulation tools combining Geant4 and TCAD are used to assess and optimize their performance. This contribution gives an overview of the R&D program for the CLIC vertex and tracking detectors, highlighting new results from the prototypes.",1812.02625v1 2019-06-22,Dynamic enlargement of a hole in a sheet: crater formation and propagation of cylindrical shock waves,"Predicting the shape of a crater formed by high velocity impact is of interest in several fields. It can aid in design of more efficient protective structures, in forensic analysis of bullet holes, and in understanding the effects of meteorite impact in both space systems and in extreme geological events. In this paper we present, for the first time, a complete theoretical solution of the dynamic plane-stress problem. We consider the steady-state expansion of a cylindrical hole in a strain hardening elastoplastic sheet and find that a self-similar field emerges if the `specific cavitation energy' is constant. It is shown that at the quasistatic limit this solution reduces to available classical solutions, while at high expansion velocities shock waves can appear. Investigation of the constitutive sensitivities of the expansion field is conducted and compared with available results for the spherical field which is commonly applied to predict resistance to high velocity penetration. It is shown that shock waves appear at significantly lower expansion velocities, in the plane-stress deformation pattern, for which material compressibility is found to have a negligible effect. This insensitivity can be taken advantage of in the future for design of light weight protective layers by incorporating porosity.",1906.09514v1 2019-10-08,Visualizing dissipative charge carrier dynamics at the nanoscale with superconducting charge qubit microscopy,"The investigation of novel electronic phases in low-dimensional quantum materials demands for the concurrent development of new measurement techniques that combine surface sensitivity with high spatial resolution and high measurement accuracy. We propose a new quantum sensing imaging modality based on superconducting charge qubits to study dissipative charge carrier dynamics with nanometer spatial and high temporal resolution. Using analytical and numerical calculations we show that superconducting charge qubit microscopy (SCQM) has the potential to resolve temperature and resistivity changes in a sample as small as $\Delta T\leq0.1\;$mK and $\Delta\rho\leq1\cdot10^{4} \,\Omega\cdot$cm, respectively. Among other applications, SCQM will be especially suited to study the microscopic mechanisms underlying interaction driven quantum phase transitions, to investigate the boundary modes found in novel topological insulators and, in a broader context, to visualize the dissiaptive charge carrier dynamics occurring in mesoscopic and nanoscale devices.",1910.03583v2 2020-06-05,Anomalous dependence of thermoelectric parameters on carrier concentration and electronic structure in Mn-substituted Fe2CrAl Heusler alloy,"We investigate the high temperature thermoelectric properties of Heusler alloys Fe2-xMnxCrAl (0 90%)",1211.5698v1 2018-06-21,Mutation rate variability as a driving force in adaptive evolution,"Mutation rate is a key determinant of the pace as well as outcome of evolution, and variability in this rate has been shown in different scenarios to play a key role in evolutionary adaptation and resistance evolution under stress caused by selective pressure. Here we investigate the dynamics of resistance fixation in a bacterial population with variable mutation rates and show that evolutionary outcomes are most sensitive to mutation rate variations when the population is subject to environmental and demographic conditions that suppress the evolutionary advantage of high-fitness subpopulations. By directly mapping a biophysical fitness function to the system-level dynamics of the population we show that both low and very high, but not intermediate, levels of stress in the form of an antibiotic result in a disproportionate effect of hypermutation on resistance fixation. We demonstrate how this behavior is directly tied to the extent of genetic hitchhiking in the system, the propagation of high-mutation rate cells through association with high-fitness mutations. Our results indicate a substantial role for mutation rate flexibility in the evolution of antibiotic resistance under conditions that present a weak advantage over wildtype to resistant cells.",1806.08454v2 2015-03-13,Paper-based spintronics: magneto-resistivity of permalloy deposited onto paper substrates,"Driven by low-cost, resource abundance and distinct material properties, the use of paper in electronics, optics and fluidics is under investigation. Considering sensor systems based on magneto-resistance principles (anisotropic, giant, tunnel) that are conventionally manufactured onto inorganic semiconductor materials, we propose the use of paper substrates for cost reduction purposes primarily. In particular, we studied the magneto-resistance sensitivity of permalloy (Py:Ni81Fe19) onto paper substrates. In this work, we report on our findings with clean room paper (80 g/m2, Rrms = 2.877 {\mu}m, 23% surface porosity, latex impregnation, no embossed macro-structure). Here, the Py:Ni81Fe19 coating was manufactured by means of a dry process, sputter deposition, and spans an area of 10x10 mm2 and a thickness of 70 nm. Employing a four-point-probe DC resistivity measurement setup, we investigated the change of electrical resistance of Py:Ni81Fe19 under the presence of an oriented external magnetic field. In particular, we investigate the magneto-resistive change at two configurations: (1) the direction of the magnetic field is parallel to the nominal induced electric current and (2) the direction of the magnetic field is perpendicular to the electric current. Due to the stochastic orientation of the fibers interplaying with the Py:Ni81Fe19 coating, the change in magneto-resistance of the overall system at both measurement configurations closely corresponds to the classical response of Py:Ni81Fe19 at a +/-45{\deg} angle between the direction of electrical current and magnetic field. Using the magneto-optic kerr effect, we observed the formation of domain walls at the fiber bending locations. Future work will focus on the impact of layer thickness, fiber dimensions and structure of magnetic coating on the performance of the paper-based Py:Ni81Fe19 magneto-resistors.",1503.04853v2 2002-12-16,"Effects of Boron Purity, Mg Stoichiometry and Carbon Substitution on Properties of Polycrystalline MgB$_{2}$","By synthesizing MgB$_{2}$ using boron of different nominal purity we found values of the residual resistivity ratio ($RRR = R(300 K) / R(42 K)$) from 4 to 20, which covers almost all values found in literature. To obtain high values of $RRR$, high purity reagents are necessary. With the isotopically pure boron we obtained the highest $RRR \sim$ 20 for the stoichiometric compound. We also investigated Mg$_{x}$$^{11}$B$_{2}$ samples with 0.8 $< x <$ 1.2. For the range Mg$_{0.8}$$^{11}$B$_{2}$ up to Mg$_{1.2}$$^{11}$B$_{2}$ we found average values of $RRR$ between 14 and 24. For smaller variations in stoichiometry ($x=1\pm 0.1$) $RRR = 18 \pm 3$. All of our data point to the conclusion that high $RRR$ ($\sim 20$) and low $\rho_{0}$ ($\leq 0.4 \mu \Omega cm$) are intrinsic material properties associated with high purity MgB$_{2}$. In addition we have performed initial work on optimizing the formation of carbon doped MgB$_{2}$ via the use of B$_{4}$C. Nearly single phase material can be formed by reaction of nominal Mg(B$_{0.8}$C$_{0.2}$)$_{2}$ for 24 hours at $1200^{\circ}C$. The $T_{c}$ for this composition is between $21.9 K$ and $22.7 K$ (depending on criterion).",0212385v1 2012-04-24,Microstructural analysis of phase separation in iron chalcogenide superconductors,"The interplay between superconductivity, magnetism and crystal structure in iron-based superconductors is a topic of great interest amongst the condensed matter physics community as it is thought to be the key to understanding the mechanisms responsible for high temperature superconductivity. Alkali metal doped iron chalcogenide superconductors exhibit several unique characteristics which are not found in other iron-based superconducting materials such as antiferromagnetic ordering at room temperature, the presence of ordered iron vacancies and high resistivity normal state properties. Detailed microstructural analysis is essential in order to understand the origin of these unusual properties. Here we have used a range of complementary scanning electron microscope based techniques, including high-resolution electron backscatter di raction mapping, to assess local variations in composition and lattice parameter with high precision and sub-micron spatial resolution. Phase separation is observed in the Csx Fe2-ySe2 crystals, with the minor phase distributed in a plate-like morphology throughout the crystal. Our results are consistent with superconductivity occurring only in the minority phase.",1204.5472v4 2017-08-16,"Single-nanowire, low-bandgap hot carrier solar cells with tunable open-circuit voltage","Compared to traditional pn-junction photovoltaics, hot carrier solar cells offer potentially higher efficiency by extracting work from the kinetic energy of photogenerated ""hot carriers"" before they cool to the lattice temperature. Hot carrier solar cells have been demonstrated in high-bandgap ferroelectric insulators and GaAs/AlGaAs heterostructures, but so far not in low-bandgap materials, where the potential efficiency gain is highest. Recently, a high open-circuit voltage was demonstrated in an illuminated wurtzite InAs nanowire with a low bandgap of 0.39 eV, and was interpreted in terms of a photothermoelectric effect. Here, we point out that this device is a hot carrier solar cell and discuss its performance in those terms. In the demonstrated devices, InP heterostructures are used as energy filters in order to thermoelectrically harvest the energy of hot electrons photogenerated in InAs absorber segments. The obtained photovoltage depends on the heterostructure design of the energy filter and is therefore tunable. By using a high-resistance, thermionic barrier an open-circuit voltage is obtained that is in excess of the Shockley-Queisser limit. These results provide generalizable insight into how to realize high voltage hot carrier solar cells in low-bandgap materials, and therefore are a step towards the demonstration of higher efficiency hot carrier solar cells.",1708.04848v1 2019-11-11,Mechanical properties of VMoNO as a function of oxygen concentration: toward development of hard and tough refractory oxynitrides,"Improved toughness is a central goal in the development of wear-resistant refractory ceramic coatings. Extensive theoretical and experimental research has revealed that NaCl structure VMoN alloys exhibit surprisingly high ductility combined with high hardness and toughness. However, during operation, protective coatings inevitably oxidize, a problem which may compromise material properties and performance. Here, we explore the role of oxidation in altering VMoN properties. Density functional theory and theoretical intrinsic hardness models are used to investigate the mechanical behavior of cubic V0.5Mo0.5N1-xOx solid solutions as a function of the oxygen concentration x. Elastic-constant and intrinsic hardness calculations show that oxidation does not degrade the mechanical properties of V0.5Mo0.5N. Electronic structure analyses indicate that the presence of oxygen reduces the covalent bond character, which slightly lowers the alloy strength and intrinsic hardness. Nevertheless, the character of metallic d-d states, which are crucial for allowing plastic deformation and enhancing toughness, remains unaffected. Overall, our results suggest that VMoNO oxynitrides, with oxygen concentrations as high as 50%, possess high intrinsic hardness, while still being ductile.",1911.04165v1 2020-12-25,Superconductivity to 262 kelvin via catalyzed hydrogenation of yttrium at high pressures,"Room temperature superconductivity has been achieved under high pressure in an organically derived carbonaceous sulfur hydride with a critical superconducting transition temperature (Tc) of 288 kelvin. This development is part of a new class of dense, hydrogen rich materials with remarkably high critical temperatures. Metal superhydrides are a subclass of these materials that provide a different and potentially more promising route to very high Tc superconductivity. The most promising binary metal superhydrides contain alkaline or rare earth elements, and recent experimental observations of LaH10 have shown them capable of Tc s up to 250 to 260 kelvin. Predictions have shown yttrium superhydrides to be the most promising with an estimated Tc in excess of 300 kelvin for YH10. Here we report the synthesis of an yttrium superhydride that exhibits superconductivity at a critical temperature of 262 kelvin at 182 gigapascal. A palladium thin film assists the synthesis by protecting the sputtered yttrium from oxidation and promoting subsequent hydrogenation. Phonon mediated superconductivity is established by the observation of zero resistance, an isotope effect and the reduction of Tc under an external magnetic field. The upper critical magnetic field is 103 tesla at zero temperature. We suggest YH9 is the synthesized product based on comparison of the measured Raman spectra and Tc to calculated Raman results.",2012.13627v1 2021-08-25,A Stable High-Capacity Lithium-Ion Battery Using a Biomass-Derived Sulfur-Carbon Cathode and Lithiated Silicon Anode,"A full lithium-ion-sulfur cell with a remarkable cycle life was achieved by combining an environmentally sustainable biomass-derived sulfur-carbon cathode and a pre-lithiated silicon oxide anode. X-ray diffraction, Raman spectroscopy, energy dispersive spectroscopy, and thermogravimetry of the cathode evidenced the disordered nature of the carbon matrix in which sulfur was uniformly distributed with a weight content as high as 75%, while scanning and transmission electron microscopy revealed the micrometric morphology of the composite. The sulfur-carbon electrode in the lithium half-cell exhibited a maximum capacity higher than 1200 mAhgS-1, reversible electrochemical process, limited electrode/electrolyte interphase resistance, and a rate capability up to C/2. The material showed a capacity decay of about 40% with respect to the steady-state value over 100 cycles, likely due to the reaction with the lithium metal of dissolved polysulfides or impurities including P detected in the carbon precursor. Therefore, the replacement of the lithium metal with a less challenging anode was suggested, and the sulfur-carbon composite was subsequently investigated in the full lithium-ion-sulfur battery employing a Li-alloying silicon oxide anode. The full-cell revealed an initial capacity as high as 1200 mAhgS-1, a retention increased to more than 79% for 100 galvanostatic cycles, and 56% over 500 cycles. The data reported herein well indicated the reliability of energy storage devices with extended cycle life employing high-energy, green, and safe electrode materials.",2108.11284v1 2023-09-07,Enhanced strength-ductility combination by introducing bimodal grains structures in high-density oxide dispersion strengthened FeCrAl alloys fabricated by spark plasma sintering technology,"Oxide dispersion strengthened FeCrAl alloys dispersed high-density nano-oxides in the matrix show outstanding corrosion resistance and mechanical properties. However, ODS FeCrAl alloys achieve the high strength generally at the expense of ductility in some way. Here, a method by introducing a bimodal grain structure was designed to overcome the strength-ductility tradeoff. In this work, ODS FeCrAl alloys were successfully fabricated through various mechanical alloying time, combined with spark plasma sintering under the vacuum of less than 4Pa. Microstructural characterization showed that the average grains size and nano-oxides size decrease gradually, and the density of nano-oxides increases, as the milling time increases. Mechanical properties revealed that both the strength and ductility were significantly synergistic enhanced with increasing milling time. The bimodal grain distribution characterized by electron backscatter diffraction (EBSD) (vacuum degree was less than 5E-5pa) was beneficial for the activation of the back stress strengthening and the annihilation of these microcracks, thus achieving the excellent ductility (27.65%). In addition, transmission electron microscope (TEM) characterization under the vacuum degree of less than 10-6pa illustrated that ultra-high-density nano-oxides (9.61E22/m3) was crucial for enhancing the strength of ODS FeCrAl alloys (993MPa). The strengthening mechanism superposition, based on the model of nano-oxides interrelated with the dislocation, illustrated an excellent agreement with experimental results from yield strength strengthening mechanisms. To our best knowledge, H40 (milled for 40h, and sintered at 1100C) alloy presents the outstanding strength with the exceptional ductility among all studied ODS FeCrAl alloys, which makes it the promising cladding materials for the accident tolerant fuel cladding.",2309.03703v1 2017-11-14,The Dominant Role of Critical Valence Fluctuations on High $T_{\rm c}$ Superconductivity in Heavy Fermions,"Despite almost 40 years of research, the origin of heavy-fermion superconductivity is still strongly debated. Especially, the pressure-induced enhancement of superconductivity in CeCu$_2$Si$_2$ away from the magnetic breakdown is not sufficiently taken into consideration. As recently reported in CeCu$_2$Si$_2$ and several related compounds, optimal superconductivity occurs at the pressure of a valence crossover, which arises from a virtual critical end point at negative temperature $T_{\rm cr}$. In this context, we did a meticulous analysis of a vast set of top-quality high-pressure electrical resistivity data of several Ce-based heavy fermion compounds. The key novelty is the salient correlation between the superconducting transition temperature $T_{\rm c}$ and the valence instability parameter $T_{\rm cr}$, which is in line with theory of enhanced valence fluctuations. Moreover, it is found that, in the pressure region of superconductivity, electrical resistivity is governed by the valence crossover, which most often manifests in scaling behavior. We develop the new idea that the optimum superconducting $T_{\rm c}$ of a given sample is mainly controlled by the compound's $T_{\rm cr}$ and limited by non-magnetic disorder. In this regard, the present study provides compelling evidence for the crucial role of critical valence fluctuations in the formation of Cooper pairs in Ce-based heavy fermion superconductors besides the contribution of spin fluctuations near magnetic quantum critical points, and corroborates a plausible superconducting mechanism in strongly correlated electron systems in general.",1711.05145v2 2017-05-09,Universal experimental test for the role of free charge carriers in thermal Casimir effect within a micrometer separation range,"We propose a universal experiment to measure the differential Casimir force between a Au-coated sphere and two halves of a structured plate covered with a P-doped Si overlayer. The concentration of free charge carriers in the overlayer is chosen slightly below the critical one, f or which the phase transition from dielectric to metal occurs. One ha f of the structured plate is insulating, while its second half is made of gold. For the former we consider two different structures, one consisting of bulk high-resistivity Si and the other of a layer of silica followed by bulk high-resistivity Si. The differential Casimir force is computed within the Lifshitz theory using four approaches that have been proposed in the literature to account for the role of free charge carriers in metallic and dielectric materials interacting with quantum fluctuations. According to these approaches, Au at low frequencies is described by either the Drude or the plasma model, whereas the free charge carriers in dielectric materials at room temperature are either taken into account or disregarded. It is shown that the values of differential Casimir forces, computed in the micrometer separation range using these four approaches, are widely distinct from each other and can be easily discriminated experimentally. It is shown that for all approaches the thermal component of the differential Casimir force is sufficiently large for direct observation. The possible errors and uncertainties in the proposed experiment are estimated and its importance for the theory of quantum fluctuations is discussed.",1705.03223v2 2021-03-10,Solid phase epitaxial growth of the correlated-electron transparent conducting oxide SrVO3,"SrVO3 thin films with a high figure of merit for applications as transparent conductors were crystallized from amorphous layers using solid phase epitaxy (SPE). Epitaxial SrVO3 films crystallized on SrTiO3 using SPE exhibit a room temperature resistivity of 2.5 x 10-5 Ohms cm, a residual resistivity ratio of 3.8, and visible light transmission above 0.5 for a 60 nm-thick film. SrVO3 layers were deposited at room temperature using radio-frequency sputtering in an amorphous form and subsequently crystallized by heating in controlled gas environment. The lattice parameters and mosaic angular width of x-ray reflections from the crystallized films are consistent with partial relaxation of the strain resulting from the epitaxial mismatch between SrVO3 and SrTiO3. A reflection high-energy electron diffraction study of the kinetics of SPE indicates that crystallization occurs via the thermally activated propagation of the crystalline/amorphous interface, similar to SPE phenomena in other perovskite oxides. Thermodynamic calculations based on density functional theory predict the temperature and oxygen partial pressure conditions required to produce the SrVO3 phase and are consistent with the experiments. The separate control of deposition and crystallization conditions in SPE presents new possibilities for the crystallization of transparent conductors in complex geometries and over large areas.",2103.05797v2 2023-11-13,Superconductivity in trilayer nickelate La$_4$Ni$_3$O$_{10}$ single crystals,"The pursuit of discovering new high-temperature superconductors that diverge from the copper-based paradigm carries profound implications for elucidating mechanisms behind superconductivity and may also enable new applications. Here, our investigation reveals that application of pressure effectively suppresses the spin and charge order in trilayer nickelate La$_4$Ni$_3$O$_{10}$ single crystals, leading to the emergence of superconductivity with a maximum critical temperature (Tc) of around 30 K. In the normal state, we observe a ""strange metal"" behavior, characterized by a linear temperature-dependent resistance extending up to 300 K. These results could be interpreted as the pressure's influence, inducing damping on the density-wave gap and spin order, while promoting spin fluctuations and bringing the associated flat dz2 band into close proximity with the Fermi surface. This, in turn, fosters strong correlations and ""strange metal"" behavior, thus setting the stage for the eventual emergence of superconductivity. Furthermore, the layer-dependent superconductivity observed hints at a unique interlayer coupling mechanism specific to nickelates, setting them apart from cuprates in this regard. Our findings provide crucial insights into the fundamental mechanisms underpinning superconductivity, while also introducing a new material platform to explore the intricate interplay between the spin/charge order, flat band structures, interlayer coupling, strange metal behavior and high-temperature superconductivity.",2311.07353v2 2019-02-28,3D quench modeling based on T-A formulation for high temperature superconductor CORC cables,"High temperature superconductor (HTS) (RE)Ba2Cu3Ox (REBCO) conductor on round core cable (CORC) has high current carrying capacity for high field magnet and power applications. In REBCO CORC cables, current redistribution occurs among tapes through terminal contact resistances when a local quench occurs. Therefore, the quench behaviour of CORC cable is different from single tape situation, for it is significantly affected by terminal contact resistances. To better understand the underlying physical process of local quenches in CORC cables, a new 3D multi-physics modelling tool for CORC cables is developed and presented in this paper. In this model, the REBCO tape is treated as a thin shell without thickness, and four models are coupled: T-formulation model, A-formulation model, a heat transfer model and an equivalent circuit model. The current redistribution, temperature and tape voltage of CORC cable during hot spot induced quenches are analysed using this model. The results show that the thermal stability of CORC cable can be considerably improved by reducing terminal contact resistance. The minimum quench energy (MQE) increases rapidly with the reduction of terminal contact resistance when the resistance is in a middle range. When the terminal contact resistance is too low or too high, the MQE shows no obvious variation with terminal contact resistances. With a low terminal contact resistance, a hot spot in one tape may induce an over-current quench on the other tapes without hot spots. This will not happen in a cable with high terminal contact resistance. In this case, the tape with hot spot will quench and burn out before inducing a quench on other tapes. The modelling tool developed can be used to design CORC cables with improved thermal stability.",1902.11055v1 2001-06-20,Saturation of electrical resistivity in metals at large temperatures,"We present a microscopic model for systems showing resistivity saturation. An essentially exact quantum Monte-Carlo calculation demonstrates that the model describes saturation. We give a simple explanation for saturation, using charge conservation and considering the limit where thermally excited phonons have destroyed the periodicity. Crucial model features are phonons coupling to the hopping matrix elements and a unit cell with several atoms. We demonstrate the difference to a model of alkali-doped C60 with coupling to the level positions, for which there is no saturation.",0106397v2 2002-05-13,Pseudogap effects on the charge dynamics in the underdoped copper oxide materials,"Within the t-J model, the charge dynamics of copper oxide materials in the underdoped regime is studied based on the fermion-spin theory. It is shown that both in-plane charge dynamics and c-axis charge dynamics are mainly governed by the scattering from the in-plane fluctuation, which would be suppressed when the holon pseudogap opens at low temperatures, leading to the temperature linear to the nonlinear range in the in-plane resistivity and crossovers to the semiconducting-like range in the c-axis resistivity.",0205248v1 2004-05-26,An Inhomogeneous Josephson Phase Near the (Super) Conductor-Insulator Transition,"In many cases inhomogeneities are known to exist near the metal (or superconductor)- insulator transition, as follows from well-known domain-wall arguments. If the conducting regions are large enough, and if they have superconducting correlations, it becomes energetically favorable for the system to go into a Josephson- coupled zero-resistance state before (i.e. at higher resistance than) the material becomes a real metal. We show that this is plausible by a simple comparison of the relevant coupling constants. We also illustrate using data in the literature on oxide materials as well as ultra-thin films, that when this proposed Josephson state is quenched by a magnetic field, an insulating, rather then a metallic, state indeed appears.",0405625v1 2005-08-15,Electronic structure and anisotropic transport properties in hexagonal YPtIn and LuAgGe ternary compounds,"We present anisotropic, zero applied magnetic field, temperature dependent resistivity measurements on hexagonal, non-magnetic, YPtIn and LuAgGe single crystals. For these materials the in-plane resistivity, $\rho_{ab}$, is significantly higher than the $c$ - axis one, $\rho_c$, with $\rho_{ab}/\rho_c \approx 1.4$ for YPtIn and $\approx 4.2 - 4.7$ for LuAgGe. The connection between the electronic structure and the anisotropic transport properties is discussed using density functional calculations that link the observed anisotropy with a specific shape of Fermi surface and anisotropy of the Fermi velocities.",0508346v1 2010-11-12,Microwave inductance of thin metal strips,"We have measured the frequency-dependent, complex impedance of thin metal strips in a broad range of microwave frequencies (45~MHz to 20~GHz). The spectra are in good agreement with theoretical predictions of an RCL model. The resistance, inductance, and capacitance, which govern the microwave response, depend on the strip width and thickness as well as on the strip and substrate materials. While the strip resistance scales inversely with the cross section, the inductance depends on the width of the strip, but not on the thickness (in the limit of small thickness).",1011.2913v1 2011-01-24,Graded anharmonic crystals as genuine thermal diodes: Analytical description of rectification and negative differential thermal resistance,"We address the heat flow study starting from microscopic models of matter: we develop an approach and investigate some anharmonic graded mass crystals, with weak interparticle interactions. We calculate the thermal conductivity, and show the existence of rectification and negative differential thermal resistance. Our formalism allows us to understand the mechanism behind the phenomena, and shows that the properties of graded materials make them genuine thermal diodes.",1101.4589v1 2011-07-15,Enhanced Gas-Flow-Induced Voltage in Graphene,"We show by systemically experimental investigation that gas-flow-induced voltage in monolayer graphene is more than twenty times of that in bulk graphite. Examination over samples with sheet resistances ranging from 307 to 1600 {\Omega}/sq shows that the induced voltage increase with the resistance and can be further improved by controlling the quality and doping level of graphene. The induced voltage is nearly independent of the substrate materials and can be well explained by the interplay of Bernoulli's principle and the carrier density dependent Seebeck coefficient. The results demonstrate that graphene has great potential for flow sensors and energy conversion devices.",1107.3049v1 2016-02-17,On the analysis of stage I in the resistivity recovery of electron irradiated iron,"The experimental results of Takaki et al. [1] on the stage I resistivity recovery of electron irradiated iron are analyzed using the analytical theory of diffusion annealing formulated by Simpson & Sossin [2] and Schroeder [3] taking into account the recent first-principles calculations of Fu et al. [4] regarding the mobility of interstitials. Excellent agreement between theory and experiment is obtained by a minimal set of adjustable parameters. The results show that the diffusion annealing equations can be successfully employed for the analysis of recovery experiments in iron.",1602.05449v2 2016-04-18,Large thermopower in the antiferromagnetic semiconductor BaMn$_2$Bi$_2$,"We report electrical and thermal transport properties of Mn-based material BaMn$_2$Bi$_2$ with ThCr$_2$Si$_2$ structure. The resistivity of the antiferromagnetic BaMn$_2$Bi$_2$ shows a metal-semiconductor transition at $\sim 80$ K with decreasing temperature. Correspondingly, the thermopower $S$ shows a peak at the same temperature, approaching ~150 $\mu$V/K. With increasing temperature $S$ decreases to about 125 $\mu$V/K at the room temperature. The magnetic field enhances the peak value to 210 $\mu$V/K. The Hall resistivity reveals an abrupt change of the carrier density close to the metal-semiconductor transition temperature.",1604.05296v1 2016-06-20,Resistivity scaling in metallic thin films and nanowires due to grain boundary and surface roughness scattering,"A modeling approach, based on an analytical solution of the semiclassical multi-subband Boltzmann transport equation, is presented to study resistivity scaling in metallic thin films and nanowires due to grain boundary and surface roughness scattering. While taking into account the detailed statistical properties of grains, roughness and barrier material as well as the metallic band structure and quantum mechanical aspects of scattering and confinement, the model does not rely on phenomenological fitting parameters.",1606.05972v2 2016-07-27,Alloy-like behaviour of the thermal conductivity of non-symmetric superlattices,"In this work, we show a phenomenological alloy-like fit of the thermal conductivity of (A)d1:(B)d2 superlattices with d1 /= d2, i.e. non-symmetric structure. The presented method is a generalization of the Norbury rule of the summation of thermal resistivities in alloy compounds. Namely, we show that this approach can be also extended to describe the thermal properties of crystalline and ordered-system composed by two or more elements, and, has a potentially much wider application range. Using this approximation we estimate that the interface thermal resistance depends on the period and the ratio of materials that form the superlattice structure",1607.08017v2 2018-03-30,Nanostructured Ceramic Oxides with a Slow Crack Growth Resistance Close to Covalent Materials,"Oxide ceramics are sensitive to slow crack growth because adsorption of water can take place at the crack tip, leading to a strong decrease of the surface energy in humid (or air) conditions. This is a major drawback concerning demanding, long-term applications such as orthopaedic implants. Here we show that a specific nanostructuration of ceramic oxides can lead to a crack resistance never reached before, similar to that of covalent ceramics.",1804.01393v1 2018-05-30,Interface thermal behavior in nanomaterials by thermal grating relaxation,"We study the relaxation of a thermal grating in multilayer materials with interface thermal resistances. The analytical development allows for the nu- merical determination of this thermal property in Approach to Equilibrium Molecular Dynamics and suggests an experimental setup for its measurement. Possible non-diffusive effects at the nanoscale are take into consideration by a non-local formulation of the heat equation. As a case study, we numerically apply the present approach to silicon grain boundary thermal resistance",1805.12086v1 2019-07-04,Pressure-induced superconductivity in SnSb2Te4,"We report the discovery of a new superconductor from phase change materials SnSb2Te4. Single crystals of SnSb2Te4 were grown using a conventional melting-growth method. The sample resistance under pressure was measured using an originally designed diamond anvil cell with boron-doped diamond electrodes. The pressure dependence of the resistance has been measured up to 32.6 GPa. The superconducting transition of SnSb2Te4 appeared at 2.1 K(Tconset) under 8.1 GPa, which was further increased with applied pressure to a maximum onset transition temperature 7.4K under 32.6 GPa.",1907.02381v1 2019-04-13,Giant Interfacial Thermal Resistance Arising From Materials With Mismatched Phonon Structures,"Previous researches only reported very small interfacial thermal resistances at room temperature due to limitations in sample combinations and methods. Taking cognizance of the importance of mismatched phonon structures, we report values up to $2*10^{-4}W^{-1}m^{2}K$, thousand times larger than highest values reported to date. This enables substantial tuning of the thermal conductivity in composites, and does not constrain other characteristics. Our findings inspire new design strategies, for heat control in integrated circuits and thermoelectric composites, that harness thermal transport at interfaces.",1904.06540v2 2020-01-26,Pulse percolation conduction and multi-value memory,"We develop a theory of pulse conduction in percolation type of materials such as noncrystalline semiconductors and nano-metal compounds. For short voltage pulses, the corresponding electric currents are inversely proportional to the pulse length and exhibit significant nonohmicity due to strong local fields in resistive regions of the percolation bonds. These fields can trigger local switching events incrementally changing bond resistances in response to pulse trains. Our prediction opens a venue to a class of multi-value nonvolatile memory implementable with a variety of materials.",2001.09512v3 2020-08-27,Nitrobenzene as Additive to Improve Reproducibility and Degradation Resistance of Highly Efficient Methylammonium-Free Inverted Perovskite Solar Cells,"We show that the addition of 1 % (v/v) nitrobenzene within the perovskite formulation can be used as a method to improve the power conversion efficiency and reliability performance of methylammonium-free (CsFA) inverted perovskite solar cells. Addition of nitrobenzene increased PCE due to defect passivation and provides smoother films resulting in PVSCs with narrower PCE distribution. Moreover, the nitrobenzene additive methylammonium-free hybrid PVSCs exhibit prolonged lifetime compare to additive free PVSCs due to enhanced air and moisture degradation resistance.",2008.12041v1 2021-10-27,Planar Hall effect in Cu intercalated PdTe$_2$,"We present the Planar Hall effect studies on the Cu intercalated type-II Dirac semimetal PdTe$_{2}$. The electrical resistivity exhibits a positive field dependence both in perpendicular and parallel field directions, causing non-zero anisotropy. The longitudinal magnetoresistance shows almost linear field dependence at low temperatures. A tilted prolate spheroid shaped orbits are observed in parametric plot between transverse and longitudinal resistivities. Our study suggest that for the type-II Dirac semimetal materials with positive longitudinal magnetoresistance, the origin of Planar Hall effect cannot be asserted with certainty to the topological or non-topological without taking into account the anisotropy of Fermi surface.",2110.14251v1 2023-10-04,Anisotropic transport and Negative Resistance in a polycrystalline metal-semiconductor (Ni-TiO2) hybrid,"We investigate anomalous electrical transport properties of a Ni-TiO2 hybrid system displaying a unique nanostructured morphology. The system undergoes an insulator to metal transition below 150 K with a low temperature metallic phase that shows negative resistance in a four-probe configuration. Temperature dependent transport measurements and numerical modelling show that the anomalies originate from the dendritic architecture of the TiO2 backbone interspersed with Ni nanoparticles that paradoxically renders this polycrystalline, heterogeneous system highly anisotropic. The study critiques inferences that may be drawn from four-probe transport measurements and offers valuable insights into modelling conductivity of anisotropic hybrid materials.",2310.02976v1 2024-02-21,Nonlinear longitudinal current of band-geometric origin in wires of finite thickness,"The miniaturization of integrated circuits is facing an obstruction due to the escalating electrical resistivity of conventional copper interconnects. The underlying reason for this problem was unveiled by Fuchs and Sondheimer, who showed that thinner wires are more resistive because current-carrying electrons encounter the rough surfaces of the wire more frequently therein. Here, we present a generalization of the Fuchs-Sondheimer theory to Dirac and Weyl materials, which are candidates for next-generation interconnects. We predict a nonlinear longitudinal electric current originating from the combined action of the Berry curvature and non-specular surface-scattering.",2402.14112v1 2007-09-25,Quantum to Classical Transition of the Charge Relaxation Resistance of a Mesoscopic Capacitor,"We present an analysis of the effect of dephasing on the single channel charge relaxation resistance of a mesoscopic capacitor in the linear low frequency regime. The capacitor consists of a cavity which is via a quantum point contact connected to an electron reservoir and Coulomb coupled to a gate. The capacitor is in a perpendicular high magnetic field such that only one (spin polarized) edge state is (partially) transmitted through the contact. In the coherent limit the charge relaxation resistance for a single channel contact is independent of the transmission probability of the contact and given by half a resistance quantum. The loss of coherence in the conductor is modeled by attaching to it a fictitious probe, which draws no net current. In the incoherent limit one could expect a charge relaxation resistance that is inversely proportional to the transmission probability of the quantum point contact. However, such a two terminal result requires that scattering is between two electron reservoirs which provide full inelastic relaxation. We find that dephasing of a single edge state in the cavity is not sufficient to generate an interface resistance. As a consequence the charge relaxation resistance is given by the sum of one constant interface resistance and the (original) Landauer resistance. The same result is obtained in the high temperature regime due to energy averaging over many occupied states in the cavity. Only for a large number of open dephasing channels, describing spatially homogenous dephasing in the cavity, do we recover the two terminal resistance, which is inversely proportional to the transmission probability of the QPC. We compare different dephasing models and discuss the relation of our results to a recent experiment.",0709.3956v1 2007-01-23,Silicon Sensors implemented on p-type substrates for high radiation resistance applications,"Silicon based micropattern detectors are essential elements of modern high energy physics experiments. Cost effectiveness and high radiation resistance are two important requirements for technologies to be used in inner tracking devices. Processes based on p-type substrates have very strong appeal for these applications. Recent results and prototype efforts under way are reviewed.",0701270v1 2021-05-01,Ultra-stable shear jammed granular material,"Dry granular materials such as sand, gravel, pills, or agricultural grains, can become rigid when compressed or sheared. At low density, one can distort the shape of a container of granular material without encountering any resistance. Under isotropic compression, the material will reach a certain {\it jamming} density and then resist further compression. {\em Shear jamming} occurs when resistance to shear emerges in a system at a density lower than the jamming density, and the elastic properties of such states have important implications for industrial and geophysical processes. We report on experimental observations of changes in the mechanical properties of a shear-jammed granular material subjected to small-amplitude, quasi-static cyclic shear. We study a layer of plastic discs confined to a shear cell, using photoelasticimetry to measure all inter-particle vector forces. For sufficiently small cyclic shear amplitudes and large enough initial shear, the material evolves to an unexpected ""ultra-stable"" state in which all the particle positions and inter-particle contact forces remain unchanged after each complete shear cycle for thousands of cycles. The stress response of these states to small imposed shear is nearly elastic, in contrast to the original shear jammed state.",2105.00313v3 2014-09-05,"Thermalization and possible quantum relaxation times in ""classical"" fluids: theory and experiment","Quantum effects in material systems are often pronounced at low energies and become insignificant at high temperatures. We find that, perhaps counterintuitively, certain quantum effects may follow the opposite route and become sharp when extrapolated to high temperature within a ""classical"" liquid phase. In the current work, we suggest basic quantum bounds on relaxation (and thermalization) times, examine kinetic theory by taking into account such possible fundamental quantum time scales, find new general equalities connecting semi-classical dynamics and thermodynamics to Planck's constant, and compute current correlation functions. Our analysis suggests that, on average, the extrapolated high temperature dynamical viscosity of general liquids may tend to a value set by the product of the particle number density ${\sf n}$ and Planck's constant $h$. We compare this theoretical result with experimental measurements of an ensemble of 23 metallic fluids where this seems to indeed be the case. The extrapolated high temperature viscosity of each of these liquids $\eta$ divided (for each respective fluid by its value of ${\sf n} h$) veers towards a Gaussian with an ensemble average value that is close to unity up to an error of size $0.6 \%$. Inspired by the Eigenstate Thermalization Hypothesis, we suggest a relation between the lowest equilibration temperature to the melting or liquidus temperature and discuss a possible corollary concerning the absence of finite temperature ""ideal glass"" transitions. We suggest a general quantum mechanical derivation for the viscosity of glasses at general temperatures. We invoke similar ideas to discuss other transport properties and demonstrate how simple behaviors including resistivity saturation and linear $T$ resistivity may appear very naturally. Our approach suggests that minimal time lags may be present in fluid dynamics.",1409.1915v14 2002-02-15,Resistance and Resistance Fluctuations in Random Resistor Networks Under Biased Percolation,"We consider a two-dimensional random resistor network (RRN) in the presence of two competing biased percolations consisting of the breaking and recovering of elementary resistors. These two processes are driven by the joint effects of an electrical bias and of the heat exchange with a thermal bath. The electrical bias is set up by applying a constant voltage or, alternatively, a constant current. Monte Carlo simulations are performed to analyze the network evolution in the full range of bias values. Depending on the bias strength, electrical failure or steady state are achieved. Here we investigate the steady-state of the RRN focusing on the properties of the non-Ohmic regime. In constant voltage conditions, a scaling relation is found between $/_0$ and $V/V_0$, where $$ is the average network resistance, $_0$ the linear regime resistance and $V_0$ the threshold value for the onset of nonlinearity. A similar relation is found in constant current conditions. The relative variance of resistance fluctuations also exhibits a strong nonlinearity whose properties are investigated. The power spectral density of resistance fluctuations presents a Lorentzian spectrum and the amplitude of fluctuations shows a significant non-Gaussian behavior in the pre-breakdown region. These results compare well with electrical breakdown measurements in thin films of composites and of other conducting materials.",0202268v1 2007-03-29,Magnetic-field cycling induced anomalous irreversibility in resistivity of charge-ordered manganites,"The rare-earth ions (RE = Eu, Dy Ho, Tm, Y) substituted charge-ordered antiferromagnetic manganites, Pr0.45RE0.05Ca0.5MnO3, were studied for the magnetic and the transport properties in the presence of external magnetic-fields of up to 14 Tesla. Regardless of the intrinsic magnetic property of RE ions, all the compounds exhibit successive step-like metamagnetic transitions at low temperatures, which are strongly correlated to their electronic transitions. At any fixed temperature in two different temperature-regimes, we observed contrary effects of the magnetic-field cycling on the resistivity of these manganites, namely, i) in the low temperature regime (<70 K), the resistivity was irreversible showing lower values than initial after a magnetic-field cycle was over, which is consistent with the irreversible magnetization, and ii) in a temperature regime above 70 K, the resistivity is irreversible with noticeably higher values than initial, whereas the magnetization was found to be reversible. For the latter case, we further show that this irreversibility of resistivity systematically depends on the temperature and the magnitude of applied magnetic-field. These results suggest that the observed resistivity behavior originated from the magnetic-field induced metamagnetic transitions and training effect.",0703771v1 2011-06-02,"Anisotropic resistivity in underdoped single crystals (Ba$_{1-x}$K$_x$)Fe$_2$As$_2$, $0 \leq x<0.35$","Temperature-dependent in-plane, $\rho_a(T)$, and inter-plane, $\rho_c(T)$, resistivities were measured for the iron-arsenide superconductor (Ba$_{1-x}$K$_x$)Fe $_2$As$_2$ over a broad doping range from parent compound to optimal doping $T_c\approx 38 K$, $0\leq x \leq 0.35$. The coupled magnetic/structural transition at $T_{SM}$ is clearly observed for samples with $T_c <$26 K ($x <0.25$), however its effect on resistivity is much weaker than in the electron-doped Ba(Fe$_{1-x}$Co$_x$)Fe $_2$As$_2$, and the transition leads only to a decrease of resistivity. In addition to the feature at $T_{SM}$, the inter-plane resistivity shows a maximum at $T^*\sim$200 K, which moves slightly to higher temperature with doping, revealing a trend opposite to the electron-doped materials. A smeared feature at about the same temperature is seen in $\rho_a(T)$. For $T 100 K with an effective moment \mu_eff = 1.82(1) \mu_B indicating an effective spin S_eff = 1/2 on the Ir^{4+} moments. A Weiss temperature \theta = - 62(1) K indicates substantial antiferromagnetic interactions between these S_eff = 1/2, Ir^{4+} moments. The \chi data in low field show a sharp cusp at T_g = 5.5 K and there is a bifurcation between zero-field-cooled (ZFC) and field-cooled (FC) data below this T. The \chi_ac data also show a sharp cusp at T_g = 5.5 K at a frequency f = 1 Hz which moves to higher temperatures with increasing f. We did not observe any anomaly at T_g in our C measurements and only a broad shoulder was observed at a much higher T = 12 K. Our results indicate that in Na_2IrO_3, a spin-glass like state occurs below the freezing temperature T_g = 5.5 K and this freezing most likely arises either from structural disorder or geometrical magnetic frustration.",1003.0973v2 2013-01-10,Micro-branching in mode-I fracture in a randomly perturbed lattice,"We study mode-I fracture in lattices with noisy bonds. In contrast to previous attempts, by using a small parameter that perturbs the force-law between the atoms in perfect lattices and using a 3-body force law, simulations reproduce the qualitative behavior of the beyond steady-state cracks in the high velocity regime, including reasonable micro-branching. As far as the physical properties such as the structure factor $g(r)$, the radial or angular distributions, these lattices share the physical properties of perfect lattices rather than that of an amorphous material (e.g., the continuous random network model). A clear transition can be seen between steady-state cracks, where a single crack propagates in the midline of the sample and the regime of unstable cracks, where micro-branches start to appear near the main crack, in line with previous experimental results. This is seen both in a honeycomb lattice and a fully hexagonal lattice. This model reproduces the main physical features of propagating cracks in brittle materials, including the behavior of velocity as a function of driving displacement and the increasing amplitude of oscillations of the electrical resistance. In addition, preliminary indications of power-law behavior of the micro-branch shapes can be seen, potentially reproducing one of the most intriguing experimental results of brittle fracture.",1301.2143v1 2013-04-24,Supramolecular Spin Valves,"Magnetic molecules possess a high potential as building blocks for the design of spintronic devices. Moreover, the use of molecular materials opens the way for the controlled use of bottom-up, e.g. supramolecular, processing techniques combining massively parallel self-fabrication with conventional top-down nanostructuring techniques. The development of solid state spintronic devices based on the giant magnetoresistance (GMR), tunnel magnetoresistance (TMR), and spin valve effects has revolutionized the field of magnetic memory applications. Recently, organic semiconductors were inserted into nanometer sized tunnel junctions allowing enhancement of spin reversal, giant magneto-resistance behaviour was observed in single non-magnetic molecules coupled to magnetic electrodes, and the use of the quantum tunnelling properties of single-molecule magnets (SMMs) in hybrid devices was proposed. Herein, we present an original device in which a non-magnetic molecular quantum dot, made of a single-wall carbon nanotube (SWCNT) contacted with non-magnetic electrodes, is laterally coupled via supramolecular interactions to a TbPc2-SMM (Pc = phthalocyanine), which provides a localized magnetic moment. The conductance through the SWCNT is modulated by sweeping the magnetic field, exhibiting magnetoresistance ratios up to 300% between fully polarized and non-polarized SMMs below 1 K. We thus demonstrate the functionality of a supramolecular spin valve without magnetic leads. Our results open up prospects of circuit-integration and implementation of new device capabilities.",1304.6543v1 2014-09-10,Controlling and distinguishing electronic transport of topological and trivial surface states in a topological insulator,"Topological insulators (TI), with characteristic Dirac-fermion topological surface states (TSS), have emerged as a new class of electronic materials with rich potentials for both novel physics and device applications. However, a major challenge with realistic TI materials is to access, distinguish and manipulate the electronic transport of TSS often obscured by other possible parallel conduction channels that include the bulk as well as a two-dimensional electron gas (2DEG) formed near the surface due to bending of the bulk bands. Such a (Schrodinger-fermion) 2DEG represents topologically-trivial surface states, whose coexistence with the TSS has been revealed by angle resolved photoemission spectroscopy. Here we show that simple manipulations of surface conditions can be used to access and control both types of surface states and their coexistence in bulk-insulating Bi2Te2Se, whose surface conduction is prominently manifested in temperature dependent resistance and nonlocal transport. The trivial 2DEG and TSS can both exhibit clear Shubnikov-de Haas oscillations in magnetoresistance, with different Berry phases ~0 and ~pi that distinguish their different topological characters. We also report a deviation from the typical weak antilocalization behavior, possibly due to high mobility TSS. Our study enables distinguishing, controlling and harnessing electronic transport of TI surface carriers with different topological natures.",1409.3217v1 2014-09-12,Fast non-thermal switching between macroscopic charge-ordered quantum states induced by charge injection,"The functionality of logic and memory elements in current electronics is based on multi-stability, driven either by manipulating local concentrations of electrons in transistors, or by switching between equivalent states of a material with a degener- ate ground state in magnetic or ferroelectric materials. Another possibility is offered by phase transitions with switching between metallic and insulating phases, but classical phase transitions are limited in speed by slow nucleation, proliferation of domains and hysteresis. We can in principle avoid these problems by using quantum states for switching, but microscopic systems suffer from decoherence which prohibits their use in everyday devices. Macroscopic quantum states, such as the superconducting ground state have the advantage that on a fundamental level they do not suffer from decoherence plaguing microscopic systems. Here we demonstrate for the first time ultrafast non-thermal switching between different metastable electronically ordered states by pulsed electrical charge injection. The macroscopic nature of the many-body quantum states(1-4) - which are not part of the equilibrium phase diagram - gives rise to unprecedented stability and remarka- bly sharp switching thresholds. Fast sub-50 ps switching, large associated re- sistance changes, 2-terminal operation and demonstrable high fidelity of bi-stability control suggest new opportunities for the use of macroscopic quantum states in electronics, particularly for an ultrafast non-volatile quantum charge-order resistive random access memory (QCOR-RAM).",1409.3794v1 2014-10-19,Enabling microstructural changes of FCC/BCC alloys in 2D dislocation dynamics,"Dimension reduction procedure is the recipe to represent defects in two dimensional dislocation dynamics according to the changes in the geometrical properties of the defects triggered by different conditions such as radiation, high temperature, or pressure. In the present study, this procedure is extended to incorporate further features related to the presence of defects with a special focus on face-centered cubic/body-centered cubic alloys used for diverse engineering purposes. In order to reflect the microstructural state of the alloy on the computational cell of two dimensional dislocation dynamics, the distribution of the multi-type defects over slip lines is implemented by using corresponding strength and line spacing for each type of defect. Additionally, a simple recursive incremental relation is set to count the loop accumulation on the precipitates. In the case of continuous resistance against the motion of edge dislocations on the slip lines, an expression of friction is introduced to see its contribution on the yield strength. Each new property is applied independently on a different material by using experimental information about defect properties and grain sizes under the condition of plain strain deformation: both constant and dynamically increasing obstacle strength for precipitate coarsening in prime-aged and heat-treated copper-chromium-zirconium, internal friction in tantalum-2.5tungsten, and mixed hardening due to the presence of precipitates and prismatic loops in irradiated oxide dispersion strengthened EUROFER with 0.3% yttria.",1410.5094v2 2015-10-22,Thermal conductivity of III-V semiconductor superlattices,"This paper presents a semiclassical model for the anisotropic thermal transport in III-V semiconductor superlattices (SLs). An effective interface rms roughness is the only adjustable parameter. Thermal transport inside a layer is described by the Boltzmann transport equation in the relaxation time approximation and is affected by the relevant scattering mechanisms (three-phonon, mass-difference, and dopant and electron scattering of phonons), as well as by diffuse scattering from the interfaces captured via an effective interface scattering rate. The in-plane thermal conductivity is obtained from the layer conductivities connected in parallel. The cross-plane thermal conductivity is calculated from the layer thermal conductivities in series with one another and with thermal boundary resistances (TBRs) associated with each interface; the TBRs dominate cross-plane transport. The TBR of each interface is calculated from the transmission coefficient obtained by interpolating between the acoustic mismatch model (AMM) and the diffuse mismatch model (DMM), where the weight of the AMM transmission coefficient is the same wavelength-dependent specularity parameter related to the effective interface rms roughness that is commonly used to describe diffuse interface scattering. The model is applied to multiple III-arsenide superlattices, and the results are in very good agreement with experimental findings. The method is both simple and accurate, easy to implement, and applicable to complicated SL systems, such as the active regions of quantum cascade lasers. It is also valid for other SL material systems with high-quality interfaces and predominantly incoherent phonon transport.",1510.06725v1 2016-08-22,Superconducting Order from Disorder in 2H-TaSe$_{2-x}$S$_{x}$ (0$\leq$x$\leq$2),"We report on the emergence of robust superconducting order in single crystal alloys of 2H-TaSe$_{2-x}$S$_{x}$ (0$\leq$x$\leq$2) . The critical temperature of the alloy is surprisingly higher than that of the two end compounds TaSe$_{2}$ and TaS$_{2}$. The evolution of superconducting critical temperature T$_{c} (x)$ correlates with the full width at half maximum of the Bragg peaks and with the linear term of the high temperature resistivity. The conductivity of the crystals near the middle of the alloy series is higher or similar than that of either one of the end members 2H-TaSe$_{2}$ and/or 2H-TaS$_{2}$. It is known that in these materials superconductivity (SC) is in close competition with charge density wave (CDW) order. We interpret our experimental findings in a picture where disorder tilts this balance in favor of superconductivity by destroying the CDW order.",1608.06275v2 2017-02-07,Quantitative Nanoscale Mapping of Three-Phase Thermal Conductivities in Filled Skutterudites via Scanning Thermal Microscopy,"In the last two decades, a nanostructuring paradigm has been successfully applied in a wide range of thermoelectric materials, resulting in significant reduction in thermal conductivity and superior thermoelectric performance. These advances, however, have been accomplished without directly investigating the local thermoelectric properties, even though local electric current can be mapped with high spatial resolution. In fact, there still lacks an effective method that links the macroscopic thermoelectric performance to the local microstructures and properties. Here, we show that local thermal conductivity can be mapped quantitatively with good accuracy, nanometer resolution, and one-to-one correspondence to the microstructure using a three-phase skutterudite as a model system. Scanning thermal microscopy combined with finite element simulations demonstrate close correlation between sample conductivity and probe resistance, enabling us to distinguish thermal conductivities spanning orders of magnitude, yet resolving thermal variation across a phase interface with small contrast. The technique thus provides a powerful tool to correlate local thermal conductivities, microstructures, and macroscopic properties for nanostructured materials in general, and nanostructured thermoelectrics in particular.",1702.01895v3 2017-06-24,Probing nanocrystalline grain dynamics in nanodevices,"Dynamical structural defects exist naturally in a wide variety of solids. They fluctuate temporally, and hence can deteriorate the performance of many electronic devices. Thus far, the entities of such dynamic objects have been identified to be individual atoms. On the other hand, it is a long-standing question whether a nanocrystalline grain constituted of a large number of atoms can switch, as a whole, reversibly like a dynamical atomic defect (i.e., a two-level system). This is an emergent issue considering the current development of nanodevices with ultralow electrical noise, qubits with long quantum coherence time, and nanoelectromechanical system (NEMS) sensors with ultrahigh resolution. Here we demonstrate experimental observations of dynamic nanocrystalline grains which repeatedly switch between two or more metastable coordinate states. We study temporal resistance fluctuations in thin ruthenium dioxide (RuO2) metal nanowires and extract microscopic parameters including relaxation time scales, mobile grain sizes, and the bonding strengths of nanograin boundaries. Such material parameters are not obtainable by other experimental approaches. When combined with previous in-situ high-resolution transmission electron microscopy (HRTEM), our electrical method can be used to infer rich information about the structural dynamics of a wide variety of nanodevices and new 2D materials.",1706.07887v1 2017-12-27,Controlled synthesis of the antiperovskite oxide superconductor Sr$_{3-x}$SnO,"A large variety of perovskite oxide superconductors are known, including some of the most prominent high-temperature and unconventional superconductors. However, superconductivity among the oxidation state inverted material class, the antiperovskite oxides, was reported just recently for the first time. In this superconductor, Sr$_{3-x}$SnO, the unconventional ionic state Sn$^{4-}$ is realized and possible unconventional superconductivity due to a band inversion has been discussed. Here, we discuss an improved facile synthesis method, making it possible to control the strontium deficiency in Sr$_{3-x}$SnO. Additionally, a synthesis method above the melting point of Sr$_{3}$SnO is presented. We show temperature dependence of magnetization and electrical resistivity for superconducting strontium deficient Sr$_{3-x}$SnO ($T_{\mathrm{c}}$ ~ 5 K) and for Sr$_{3}$SnO without a superconducting transition down to 0.15 K. Further, we reveal a significant effect of strontium raw material purity on the superconductivity and achieve 40% increased superconducting volume fraction (~100%) compared to the highest value reported so far. More detailed characterisation utilising powder X-ray diffraction and energy-dispersive X-ray spectroscopy show that a minor cubic phase, previously suggested to be a Sr$_{3-x}$SnO, is SrO. The improved characterization and controlled synthesis reported herein enable detailed investigations on the superconducting nature and its dependency on the strontium deficiency in Sr$_{3-x}$SnO.",1712.09484v1 2018-04-11,NMR and the antiferromagnetic crystal phase regions in rapidly quenched ribbons and in alloys of the type $Cu-Mn-Al$,"It was shown that anomalous resistivity behavior of the $Cu-Mn-Al$ ribbons is explained by the s-d interaction between conduction electrons and the clustered Mn atoms. While nuclear magnetic resonance measurements show the antiferromagnetic and ferromagnetic clusters of Mn atom coexisting without long-range order, it is an interesting problem to study magnetic resonance properties also for the antiferromagnetic crystal phase regions (which have long-range order for larger regions) and which may also occur in these ribbons. The Heusler Type $Cu-Mn-Al$ Alloy has a composition half way between $Cu_{2}MnAl$ and $Cu_{3}Al$. Electron microscopy of the premartensitic $\beta Cu-Zn-Al$ alloy has shown that the $\beta Cu-Zn-Al$ alloy quenched from high temperature has the electron diffraction patterns of this alloy well explained by the model with the existence of small particles with an orthorhombic structure. It was noted that an important aspect of improvement in the material properties is to create a nanostructured state in matrix, which has significant advantages in magnetic and mechanical characteristics in contrast to the bulk materials in crystalline or amorphous state. It is an interesting problem to study magnetic resonance properties not only for the Mn atoms and clusters without long-range order but also for the antiferromagnetic crystal phase regions (which have long-range order for larger regions) which may also occur in ribbons. This is the aim of our paper.",1804.04196v1 2020-03-25,Magnetic-field-induced FM-AFM metamagnetic transition and strong negative magnetoresistance in Mn$_{1/4}$NbS$_2$ under pressure,"Transition metal dichalcogenides (TMDC) stand out with their high chemical stability and the possibility to incorporate a wide range of magnetic species between the layers. The behavior of conduction electrons in such materials intercalated by 3d-elements is closely related to their magnetic properties and can be sensitively controlled by external magnetic fields. Here, we study the magnetotransport properties of NbS$_2$ intercalated with Mn, Mn$_{1/4}$NbS$_2$, demonstrating a complex behavior of the magnetoresistance and of the ordinary and anomalous Hall resistivities. Application of pressure as tuning parameter leads to the drastic changes of the magnetotransport properties of Mn$_{1/4}$NbS$_2$ exhibiting large negative magnetoresistance up to $65 \%$ at 7.1 GPa. First-principles electronic structure calculations indicates pressure-induced transition from ferromagnetic to antiferromagnetic state. Theoretical calculations accounting for the finite temperature magnetic properties of Mn$_{1/4}$NbS$_2$ suggest a field-induced metamagnetic ferromagnetic-antiferromagnetic transition as an origin of the large negative magentoresistance. These results inspire the development of materials for spintronic applications based on intercalated TMDC with a well controllable metamagnetic transition.",2003.11678v1 2017-03-16,Elemental Phosphorus: structural and superconducting phase diagram under pressure,"Pressure-induced superconductivity and structural phase transitions in phosphorous (P) are studied by resistivity measurements under pressures up to 170 GPa and fully $ab-initio$ crystal structure and superconductivity calculations up to 350 GPa. Two distinct superconducting transition temperature (T$_{c}$) vs. pressure ($P$) trends at low pressure have been reported more than 30 years ago, and for the first time we are able to reproduce them and devise a consistent explanation founded on thermodynamically metastable phases of black-phosphorous. Our experimental and theoretical results form a single, consistent picture which not only provides a clear understanding of elemental P under pressure but also sheds light on the long-standing and unsolved $anomalous$ superconductivity trend. Moreover, at higher pressures we predict a similar scenario of multiple metastable structures which coexist beyond their thermodynamical stability range. Metastable phases of P experimentally accessible at pressures above 240 GPa should exhibit T$_{c}$'s as high as 15 K, i.e. three times larger than the predicted value for the ground-state crystal structure. We observe that all the metastable structures systematically exhibit larger transition temperatures than the ground-state ones, indicating that the exploration of metastable phases represents a promising route to design materials with improved superconducting properties.",1703.05694v1 2018-10-08,Monte Carlo phonon transport simulations in hierarchically disordered silicon nanostructures,"Hierarchical material nanostructuring is considered to be a very promising direction for high performance thermoelectric materials. In this work we investigate thermal transport in hierarchically nanostructured silicon. We consider the combined presence of nanocrystallinity and nanopores, arranged under both ordered and randomized positions and sizes, by solving the Boltzmann transport equation using the Monte Carlo method. We show that nanocrystalline boundaries degrade the thermal conductivity more drastically when the average grain size becomes smaller than the average phonon mean free path. The introduction of pores degrades the thermal conductivity even further. Its effect, however, is significantly more severe when the pore sizes and positions are randomized, as randomization results in regions of higher porosity along the phonon transport direction, which introduce significant thermal resistance. We show that randomization acts as a large increase in the overall effective porosity. Using our simulations, we show that existing compact nanocrystalline and nanoporous theoretical models describe thermal conductivity accurately under uniform nanostructured conditions, but overestimate it in randomized geometries. We propose extensions to these models that accurately predict the thermal conductivity of randomized nanoporous materials based solely on a few geometrical features. Finally, we show that the new compact models introduced can be used within Matthiessens rule to combine scattering from different geometrical features within approximately 10 per cent accuracy.",1810.03334v1 2020-09-22,A cracking oxygen story: a new view of stress corrosion cracking in titanium alloys,"Titanium alloys can suffer from halide-associated stress corrosion cracking at elevated temperatures e.g., in jet engines, where chlorides and Ti-oxide promote the cracking of water vapour in the gas stream, depositing embrittling species at the crack tip. Here we report, using isotopically-labelled experiments, that crack tips in an industrial Ti-6Al-2Sn-4Zr-6Mo alloy are strongly enriched (>5 at.%) in oxygen from the water vapour, far greater than the amounts (0.25 at.%) required to embrittle the material. Surprisingly, relatively little hydrogen (deuterium) is measured, despite careful preparation and analysis. Therefore, we suggest that a combined effect of O and H leads to cracking, with O playing a vital role, since it is well-known to cause embrittlement of the alloy. In contrast it appears that in alpha+beta Ti alloys, it may be that H may drain away into the bulk owing to its high solubility in beta-Ti, rather than being retained in the stress field of the crack tip. Therefore, whilst hydrides may form on the fracture surface, hydrogen ingress might not be the only plausible mechanism of embrittlement of the underlying matrix. This possibility challenges decades of understanding of stress-corrosion cracking as being related solely to the hydrogen enhanced localised plasticity (HELP) mechanism, which explains why H-doped Ti alloys are embrittled. This would change the perspective on stress corrosion embrittlement away from a focus purely on hydrogen to also consider the ingress of O originating from the water vapour, insights critical for designing corrosion resistant materials.",2009.10567v2 2017-05-08,"Casimir free energy of dielectric films: Classical limit, low-temperature behavior and control","The Casimir free energy of dielectric films, both free-standing in vacuum and deposited on metallic or dielectric plates, is investigated. It is shown that the values of the free energy depend considerably on whether the calculation approach used neglects or takes into account the dc conductivity of film material. We demonstrate that there are the material-dependent and universal classical limits in the former and latter cases, respectively. The analytic behavior of the Casimir free energy and entropy for a free-standing dielectric film at low temperature in found. According to our results, the Casimir entropy goes to zero when the temperature vanishes if the calculation approach with neglected dc conductivity of a film is employed. If the dc conductivity is taken into account, the Casimir entropy takes the positive value at zero temperature, depending on the parameters of a film, i.e., the Nernst heat theorem is violated. By considering the Casimir free energy of silica and sapphire films deposited on a Au plate in the framework of two calculation approaches, we argue that physically correct values are obtained by disregarding the role of dc conductivity. A comparison with the well known results for the configuration of two parallel plates is made. Finally, we compute the Casimir free energy of silica, sapphire and Ge films deposited on high-resistivity Si plates of different thicknesses and demonstrate that it can be positive, negative and equal to zero. Possible applications of the obtained results to thin films used in microelectronics are discussed.",1705.02897v1 2017-07-17,Realizing Thermoelectric and Thermistor Bi-functionalities via Triggering Electron Correlations with Lattice-dipole,"Establishing strong electron-correlations not only shed lights on overcoming the trade-off limitations for optimizing thermoelectric materials, but can also introduce new functionalities that extend the vision of conventional thermoelectric applications. Here, we demonstrate that the high thermoelectric and thermistor functionalities coexist in lattice distorted SrNbxTi1-xO3 films with electron correlations between carriers and ordering aligned lattice dipoles. As-grown SrNbxTi1-xO3/SrTiO3 with effectively preserved interfacial strains exhibits cross-plane charge ordering and orbital anisotropy, as indicated by the polarization dependent near edge X-ray absorption fine structures. The resultant coulomb-correlations regulate the carrier transport and enhance the Seebeck coefficient more independently via enlarging the system vibration entropy. As-achieved maximum thermoelectric power factor exceeds 100 uWcm-1K-2 measured in the bulk performance of SrNb0.2Ti0.8O3 (2.2 um)/SrTiO3 (100 um), which is comparable to the best thermoelectric materials for low temperature applications. In addition, the strong temperature dependence of the carrier scattering aroused by the lattice dipoles introduces a positive temperature dependent thermistor transportation behavior with large temperature coefficient of resistance ranging from 30 to 300 K, which is rarely seen in conventional thermistors. Combining both functionalities largely extend the horizon in exploring new Joule sensors for detection of temperature and thermal perturbations across a broad temperature range.",1707.04988v2 2017-08-17,Tailoring tricolor structure of magnetic topological insulator for robust axion insulator,"Exploration of novel electromagnetic phenomena is a subject of great interest in topological quantum materials. One of the unprecedented effects to be experimentally verified is topological magnetoelectric (TME) effect originating from an unusual coupling of electric and magnetic fields in materials. A magnetic heterostructure of topological insulator (TI) hosts such an exotic magnetoelectric coupling and can be expected to realize the TME effect as an axion insulator. Here we designed a magnetic TI with tricolor structure where a non-magnetic layer of (Bi, Sb)2Te3 is sandwiched by a soft ferromagnetic Cr-doped (Bi, Sb)2Te3 and a hard ferromagnetic V-doped (Bi, Sb)2Te3. Accompanied by the quantum anomalous Hall (QAH) effect, we observe zero Hall conductivity plateaus, which are a hallmark of the axion insulator state, in a wide range of magnetic field between the coercive fields of Cr- and V-doped layers. The resistance of the axion insulator state reaches as high as 10^9 ohm, leading to a gigantic magnetoresistance ratio exceeding 10,000,000% upon the transition from the QAH state. The tricolor structure of TI may not only be an ideal arena for the topologically distinct phenomena, but also provide magnetoresistive applications for advancing dissipationless topological electronics.",1708.05387v1 2019-03-02,AC Elastocaloric effect as a probe for thermodynamic signatures of continuous phase transitions,"Studying the response of materials to strain can elucidate subtle properties of electronic structure in strongly correlated materials. So far, mostly the relation between strain and resistivity, the so called elastoresistivity, has been investigated. The elastocaloric effect is a second rank tensor quantity describing the relation between entropy and strain. In contrast to the elastoresistivity, the elastocaloric effect is a thermodynamic quantity. Experimentally, elastocaloric effect measurements are demanding since the thermodynamic conditions during the measurement have to be well controlled. Here we present a technique to measure the elastocaloric effect under quasi adiabatic conditions. The technique is based on oscillating strain, which allows for increasing the frequency of the elastocaloric effect above the thermal relaxation rate of the sample. We apply the technique to Co-doped iron pnictide superconductors and show that the thermodynamic signatures of second order phase transitions in the elastocaloric effect closely follow those observed in calorimetry experiments. In contrast to the heat capacity, the electronic signatures in the elastocaloric effect are measured against a small phononic background even at high temperatures, establishing this technique as a powerful complimentary tool for extracting the entropy landscape proximate to a continuous phase transition.",1903.00791v1 2019-03-27,Investigation of Room Temperature Ferroelectricity and Ferrimagnetism in Multiferroic AlxFe2-xO3 Epitaxial Thin Films,"Multiferroic materials open up the possibility to design novel functionality in electronic devices, with low energy consumption. However, there are very few materials that show multiferroicity at room temperature, which is essential to be practically useful. AlxFe2-xO3 (x-AFO) thin films, belonging to the k-Al2O3 family are interesting because they show room temperature ferrimagnetism and have a polar crystal structure. However, it is difficult to realise its ferroelectric properties at room temperature, due to low resistivity of the films. In this work, we have deposited x-AFO (0.5 <= x <= 1) epitaxial thin films with low leakage, on SrTiO3<111> substrates by Pulsed Laser Deposition. Magnetic measurements confirmed room temperature ferrimagnetism of the films, however the Curie temperature was found to be influenced by deposition conditions. First principle calculations suggested that ferroelectric domain switching occurs through shearing of in-plane oxygen layers, and predicted a high polarization value of 24 uC/cm2. However, actual ferroelectric measurements showed the polarization to be two order less. Presence of multiple in-plane domains which oppose polarization switching of adjacent domains, was found to be the cause for the small observed polarization. Comparing dielectric relaxation studies and ferroelectric characterization showed that oxygen-vacancy defects assist domain wall motion, which in turn facilitates polarization switching.",1903.11422v1 2016-09-09,Extremely large magnetoresistance in a topological semimetal candidate pyrite PtBi2,"While pyrite-type PtBi2 with face-centered cubic structure has been predicted to be a three-dimensional (3D) Dirac semimetal, experimental study on its physical properties remains absent. Here we report the angular-dependent magnetoresistance (MR) measurements of PtBi2 single-crystal under high magnetic fields. We observed extreme large unsaturated magnetoresistance (XMR) up to 11.2 million percent at T = 1.8 K in a magnetic field of 33 T, which surpasses the previously reported Dirac materials, such as WTe2, LaSb and NbP. The crystals exhibit an ultrahigh mobility and significant Shubnikov-de Hass (SdH) quantum oscillations with nontrivial Berry's phase. Analysis of Hall resistivity indicates that the XMR can be ascribed to the nearly compensated electron and hole. Our experimental results associated with the ab initio calculations suggest that pyrite PtBi2 is a topological semimetal candidate which might provide a platform for exploring topological materials with XMR in noble metal alloys.",1609.02626v2 2019-06-19,"Apparatus for Seebeck coefficient measurement of wire, thin film and bulk materials in the wide temperature range (80-650K)","A Seebeck coefficient measurement apparatus has been designed and developed, which is very effective for accurate characterization of different type of samples in a wide temperature range (80 - 650K) simultaneously covering low as well as the high-temperature regime. Reducing the complexity of the technical design of sample holder and data collections has always been challenging to implement in a single instrument when samples are in different geometrical shape and electronic structure. Our unique design of sample holder with pressure probes covers measurements of different samples shapes (wires, thin films and pellets) as well as different resistivity ranges (metals, semiconductors and insulators). It is suitable for characterization of different samples sizes (3-12 mm). A double heater configuration powered by a dual channel source meter is employed for maintaining a desired constant temperature difference across the sample for the whole temperature range. Two K-type thermocouples are used for simultaneously reading of temperatures and Seebeck voltages by utilizing different channels of a multichannel digital multimeter. Calibration of the system has been carried out using constantan, chromel and alumel materials and recorded data is found to be very accurate and consistent with earlier reports. The Seebeck coefficients of standard samples of constantan (wire) and GaN (thin film) have been reported, which shows the measurement capability of designed setup with versatile samples.",1906.08023v2 2019-11-20,Piezoelectricity in monolayer hexagonal boron nitride,"Two-dimensional (2D) hexagonal boron nitride (hBN) is a wide-bandgap van der Waals crystal with a unique combination of properties, including exceptional strength, large oxidation resistance at high temperatures and optical functionalities. Furthermore, in recent years hBN crystals have become the material of choice for encapsulating other 2D crystals in a variety of technological applications, from optoelectronic and tunnelling devices to composites. Monolayer hBN, which has no center of symmetry, has been predicted to exhibit piezoelectric properties, yet experimental evidence is lacking. Here, by using electrostatic force microscopy, we observed this effect as a strain-induced change in the local electric field around bubbles and creases, in agreement with theoretical calculations. No piezoelectricity was found in bilayer and bulk hBN, where the centre of symmetry is restored. These results add piezoelectricity to the known properties of monolayer hBN, which makes it a desirable candidate for novel electromechanical and stretchable optoelectronic devices, and pave a way to control the local electric field and carrier concentration in van der Waals heterostructures via strain. The experimental approach used here also shows a way to investigate the piezoelectric properties of other materials on the nanoscale by using electrostatic scanning probe techniques.",1911.09134v1 2020-07-16,The influence of material properties and process parameters on the spreading process in additive manufacturing,"Laser powder bed fusion (LPBF) is an additive manufacturing (AM) technology. To achieve high product quality, the powder is best spread as a uniform, dense layer. The challenge for LPBF manufacturers is to develop a spreading process that can produce a consistent layer quality for the many powders used, which show considerable differences in spreadability. Therefore, we investigate the influence of material properties, process parameters and the type of spreading tool on the layer quality. The discrete particle method is used to simulate the spreading process and to define metrics to evaluate the powder layer characteristics. We found that particle shape and surface roughness in terms of rolling resistance and interparticle sliding friction as well as particle cohesion all have a major (sometimes surprising) influence on the powder layer quality: more irregular shaped particles, rougher particle surfaces and/or higher interfacial cohesion usually, but not always, lead to worse spreadability. Our findings illustrate that there is a trade-off between material properties and process parameters. Increasing the spreading speed decreases layer quality for non- and weakly cohesive powders, but improves it for strongly cohesive ones. Using a counter-clockwise rotating roller as a spreading tool improves the powder layer quality compared to spreading with a blade. Finally, for both geometries, a unique correlation between the quality criteria uniformity and mass fraction is reported and some of the findings are related to size-segregation during spreading.",2007.10125v1 2021-03-12,Nanodevices engineering and spin transport properties of MnBi2Te4 monolayer,"Two-dimensional (2D) magnetic materials are essential for the development of the next-generation spintronic technologies. Recently, layered van der Waals (vdW) compound MnBi2Te4 (MBT) has attracted great interest, and its 2D structure has been reported to host coexisting magnetism and topology. Here, we design several conceptual nanodevices based on MBT monolayer (MBT-ML) and reveal their spin-dependent transport properties by means of the first-principles calculations. The pn-junction diodes and sub-3-nm pin-junction field-effect transistors (FETs) show a strong rectifying effect and a spin filtering effect, with an ideality factor n close to 1 even at a reasonably high temperature. In addition, the pip- and nin-junction FETs give an interesting negative differential resistive (NDR) effect. The gate voltages can tune currents through these FETs in a large range. Furthermore, the MBT-ML has a strong response to light. Our results uncover the multifunctional nature of MBT-ML, pave the road for its applications in diverse next-generation semiconductor spin electric devices.",2103.07025v1 2021-04-12,Fiber Packing and Morphology Driven Moisture Diffusion Mechanics in Reinforced Composites,"Fiber reinforced polymer composite (FRPC) materials are extensively used in lightweight applications due to their high specific strength and other favorable properties including enhanced endurance and corrosion resistance. However, these materials are inevitably exposed to moisture, which is known to drastically reduce their mechanical properties caused by moisture absorption and often accompanied with plasticization, weight gain, hygrothermal swelling, and de-bonding between fiber and matrix. Hence, it is vital to understand moisture diffusion mechanics into FRPCs. The presence of fibers, especially impermeable like Carbon fibers, introduce tortuous moisture diffusion pathways through polymer matrix. In this paper, we elucidate the impact of fiber packing and morphology on moisture diffusion in FRPC materials. Computational models are developed within a finite element framework to evaluate moisture kinetics in impermeable FRPCs. We introduce a tortuosity factor for measuring the extent of deviation in moisture diffusion pathways due to impermeable fiber reinforcements. Two-dimensional micromechanical models are analyzed with varying fiber volume fractions, spatial distributions and morphology to elucidate the influence of internal micromechanical fiber architectures on tortuous diffusion pathways and corresponding diffusivities. Finally, a relationship between tortuosity and diffusivity is established such that diffusivity can be calculated using tortuosity for a given micro-architecture. Tortuosity can be easily calculated for a given architecture by solving steady state diffusion governing equations, whereas time-dependent transient diffusion equations need to be solved for calculating moisture diffusivity. Hence, tortuosity, instead of diffusivity, can be used in future composites designs, multi-scale analyses, and optimization for enabling robust structures in moisture environments.",2104.05180v2 2021-05-01,Anisotropy and Current Control of Magnetization in SrRuO$_3$ SrTiO$_3$ Heterostructures for Spin-Memristors,"Spintronics-based nonvolatile components in neuromorphic circuits offer the possibility of realizing novel functionalities at low power. Current-controlled electrical switching of magnetization is actively researched in this context. Complex oxide heterostructures with perpendicular magnetic anisotropy (PMA), consisting of SrRuO$_3$ (SRO) grown on SrTiO$_3$ (STO) are strong material contenders. Utilizing the crystal orientation, magnetic anisotropy in such simple heterostructures can be tuned to either exhibit a perfect or slightly tilted PMA. Here, we investigate current-induced magnetization modulation in such tailored ferromagnetic layers with a material with strong spin-orbit coupling (Pt), exploiting the spin Hall effect. We find significant differences in the magnetic anisotropy between the SRO/STO heterostructures, as manifested in the first and second harmonic magnetoresistance measurements. Current-induced magnetization switching can be realized with spin-orbit torques, but for systems with perfect PMA this switching is probabilistic as a result of the high symmetry. Slight tilting of the PMA can break this symmetry and allow the realization of deterministic switching. Control over the magnetic anisotropy of our heterostructures therefore provides control over the manner of switching. Based on our findings, we propose a three-terminal spintronic memristor, with a magnetic tunnel junction design, that shows several resistive states controlled by electric charge. Non-volatile states can be written through SOT by applying an in-plane current, and read out as a tunnel current by applying a small out-of-plane current. Depending on the anisotropy of the SRO layer, the writing mechanism is either deterministic or probabilistic allowing for different functionalities to emerge. We envisage that the probabilistic MTJs could be used as synapses while the deterministic devices can emulate neurons",2105.00269v1 2021-05-05,Ni$_{80}$Fe$_{20}$ Nanotubes with Optimized Spintronic Functionalities Prepared by Atomic Layer Deposition,"Permalloy Ni$_{80}$Fe$_{20}$ is one of the key magnetic materials in the field of magnonics. Its potential would be further unveiled if it could be deposited in three dimensional (3D) architectures of sizes down to the nanometer. Atomic Layer Deposition, ALD, is the technique of choice for covering arbitrary shapes with homogeneous thin films. Early successes with ferromagnetic materials include nickel and cobalt. Still, challenges in depositing ferromagnetic alloys reside in the synthesis via decomposing the consituent elements at the same temperature and homogeneously. We report plasma-enhanced ALD to prepare permalloy Ni$_{80}$Fe$_{20}$ thin films and nanotubes using nickelocene and iron(III) tert-butoxide as metal precursors, water as the oxidant agent and an in-cycle plasma enhanced reduction step with hydrogen. We have optimized the ALD cycle in terms of Ni:Fe atomic ratio and functional properties. We obtained a Gilbert damping of 0.013, a resistivity of 28 $\mu\Omega$cm and an anisotropic magnetoresistance effect of 5.6 $\%$ in the planar thin film geometry. We demonstrate that the process also works for covering GaAs nanowires, resulting in permalloy nanotubes with high aspect ratios and diameters of about 150 nm. Individual nanotubes were investigated in terms of crystal phase, composition and spin-dynamic response by microfocused Brillouin Light Scattering. Our results enable NiFe-based 3D spintronics and magnonic devices in curved and complex topology operated in the GHz frequency regime.",2105.01969v1 2021-09-17,Towards replacing physical testing of granular materials with a Topology-based Model,"In the study of packed granular materials, the performance of a sample (e.g., the detonation of a high-energy explosive) often correlates to measurements of a fluid flowing through it. The ""effective surface area,"" the surface area accessible to the airflow, is typically measured using a permeametry apparatus that relates the flow conductance to the permeable surface area via the Carman-Kozeny equation. This equation allows calculating the flow rate of a fluid flowing through the granules packed in the sample for a given pressure drop. However, Carman-Kozeny makes inherent assumptions about tunnel shapes and flow paths that may not accurately hold in situations where the particles possess a wide distribution in shapes, sizes, and aspect ratios, as is true with many powdered systems of technological and commercial interest. To address this challenge, we replicate these measurements virtually on micro-CT images of the powdered material, introducing a new Pore Network Model based on the skeleton of the Morse-Smale complex. Pores are identified as basins of the complex, their incidence encodes adjacency, and the conductivity of the capillary between them is computed from the cross-section at their interface. We build and solve a resistive network to compute an approximate laminar fluid flow through the pore structure. We provide two means of estimating flow-permeable surface area: (i) by direct computation of conductivity, and (ii) by identifying dead-ends in the flow coupled with isosurface extraction and the application of the Carman-Kozeny equation, with the aim of establishing consistency over a range of particle shapes, sizes, porosity levels, and void distribution patterns.",2109.08777v1 2021-11-11,Tuning the Room Temperature Ferromagnetism in Fe5GeTe2 by Arsenic Substitution,"In order to tune the magnetic properties of the cleavable high-Curie temperature ferromagnet Fe$_{5-x}$GeTe$_2$, the effect of increasing the electron count through arsenic substitution has been investigated. Small additions of arsenic (2.5 and 5%) seemingly enhance ferromagnetic order in polycrystalline samples by quenching fluctuations on one of the three magnetic sublattices, whereas larger As concentrations decrease the ferromagnetic Curie temperature ($T_{\rm C}$) and saturation magnetization. This work also describes the growth and characterization of Fe$_{4.8}$AsTe$_2$ single crystals that are structurally analogous to Fe$_{5-x}$GeTe$_2$ but with some phase stability complications. Magnetization measurements reveal dominant antiferromagnetic behavior in Fe$_{4.8}$AsTe$_2$ with a N\'{e}el temperature of $T_{\rm N}$ $\approx$42K. A field-induced spin-flop below $T_{\rm N}$ results in a switch from negative to positive magnetoresistance, with significant hysteresis causing butterfly-shaped resistance loops. In addition to reporting the properties of Fe$_{4.8}$AsTe$_2$, this work shows the importance of manipulating the individual magnetic sublattices in Fe$_{5-x}$GeTe$_2$ and motivates further efforts to control the magnetic properties in related materials by fine tuning of the Fermi energy or crystal chemistry.",2111.06439v1 2022-01-11,Antiferromagnetic Excitonic Insulator State in Sr3Ir2O7,"Excitonic insulators are usually considered to form via the condensation of a soft charge mode of bound electron-hole pairs. This, however, presumes that the soft exciton is of spin-singlet character. Early theoretical considerations have also predicted a very distinct scenario, in which the condensation of magnetic excitons results in an antiferromagnetic excitonic insulator state. Here we report resonant inelastic x-ray scattering (RIXS) measurements of Sr3Ir2O7. By isolating the longitudinal component of the spectra, we identify a magnetic mode that is well-defined at the magnetic and structural Brillouin zone centers, but which merges with the electronic continuum in between these high-symmetry points and which decays upon heating concurrent with a decrease in the material's resistivity. We show that a bilayer Hubbard model, in which electron-hole pairs are bound by exchange interactions, consistently explains all the electronic and magnetic properties of Sr3Ir2O7 indicating that this material is a realization of the long-predicted antiferromagnetic excitonic insulators phase.",2201.04030v1 2022-03-18,Surface temperature and emissivity measurement for materials exposed to a flame through two-color IR-thermography,"Two-color (2C) pyrometry has long been used for flame temperature and soot concentration studies and is now becoming more widely used to measure surface temperatures of burning materials. With the obvious advantage of being a contact-free method that requires only minimal optical access, 2C pyrometry combined with high-speed acquisition is a promising diagnostic tool to obtain exceptional temporal and spatial resolution of thermally degrading samples. However, its conceptual simplicity relies on a set of basic assumptions that when violated can result in large errors. In this work, we use an experimental configuration representative for fire resistance testing for aerospace and naval applications to analyze the impact of camera parameters and test setup on the accuracy of the surface temperature results obtained. Two types of fibre reinforced polymer composites and a steel plate are used to investigate material specific aspects that effect the measurements. An improved workflow for camera calibration is presented that takes the actual experimental setup into account. The temperature and emissivity mapping obtained trough in-situ IR measurements is compared against data acquired trough thermocouples and post-fire hemispherical directional reflectance measurements at room temperature. This comparison illustrates the necessity for proper post-processing and demonstrates that emissivity values obtained from pristine or burnt samples are not well suited to obtain accurate surface temperatures through conventional (single color) IR thermography. We also present a detailed error budget and suggestions for calibration measurements to keep the overall error well below 50 K in a temperature range from 673 K - 1473 K.",2203.09689v1 2022-04-11,A-type antiferromagnetic order in semiconducting EuMg$_2$Sb$_2$ single crystals,"Eu-based Zintl-phase materials EuA$_2$Pn$_2$ (A = Mg, In, Cd, Zn; Pn = Bi, Sb, As, P) have generated significant recent interest owing to the complex interplay of magnetism and band topology. Here, we investigated the electronic, magnetic, and electronic properties of the layered Zintl-phase single crystals of EuMg$_2$Sb$_2$ with the trigonal CaAl$_2$Si$_2$ crystal structure (space group $P\bar{3}m1$). Electrical resistivity measurements complemented with angle-resolved photoemission spectroscopy (ARPES) studies find an activated behavior with the intrinsic conductivity at high temperatures indicating a semiconducting electronic ground state with a narrow energy gap of 370 meV. Magnetic susceptibility and zero-field heat-capacity measurements indicate that the compound undergoes antiferromagnetic (AFM) ordering at the Neel temperature $T_{\rm N}$ = 8.0(2) K. Zero-field neutron-diffraction measurements reveal that the AFM ordering is A-type where the Eu ordered moments (Eu$^{2+}$, S= 7/2) arranged in ab-plane layers are aligned ferromagnetically in the ab plane with the Eu moments in adjacent layers aligned antiferromagnetically. We also find that Eu-moment reorientation in the trigonal AFM domains within the ab planes occurs below $T_{\rm N}$ at low fields < 0.05 T due to very small in-plane anisotropy. Although isostructural semimetallic EuMg$_2$Bi$_2$ is reported to host Dirac surface states, the observation of narrow-gap semiconducting behavior in EuMg$_2$Sb$_2$ implies a strong role of spin-orbit coupling in tuning the electronic states of these materials.",2204.05261v1 2022-05-11,Tunable photochemical deposition of silver nanostructures on layered ferroelectric CuInP$_2$S6,"2D layered ferroelectric materials such as CuInP$_2$S6 (CIPS) are promising candidates for novel and high-performance photocatalysts, owning to their ultrathin layer thickness, strong interlayer coupling, and intrinsic spontaneous polarization, while how to control the photocatalytic activity in layered CIPS remains unexplored. In this work, we report for the first time the photocatalytic activity of ferroelectric CIPS for the chemical deposition of silver nanostructures (AgNSs). The results show that the shape and spatial distribution of AgNSs on CIPS are tunable by controlling layer thickness, environmental temperature, and light wavelength. The ferroelectric polarization in CIPS plays a critical role in tunable AgNS photodeposition, as evidenced by layer thickness and temperature dependence experiments. We further reveal that AgNS photodeposition process starts from the active site creation, selective nanoparticle nucleation/aggregation, to the continuous film formation. Moreover, AgNS/CIPS heterostructures prepared by photodeposition exhibit excellent resistance switching behavior and good surface enhancement Raman Scattering activity. Our findings provide new insight into the photocatalytic activity of layered ferroelectrics and offer a new material platform for advanced functional device applications in smart memristors and enhanced chemical sensors.",2205.05385v2 2022-06-23,Superconductivity in the crystallogenide LaFeSiO$_{1-δ}$ with squeezed FeSi layers,"Pnictogens and chalcogens are both viable anions for promoting Fe-based superconductivity and intense research activity in the related families has established systematic correlation between the Fe-anion height and the superconducting critical temperature $T_c$, with an optimum Fe-anion height of $\sim$ 1.38 \r{A}. Here, we report the discovery of superconductivity in a novel compound LaFeSiO$_{1-\delta}$ that incorporates a crystallogen element, Si, and challenges the above picture: considering the strongly squeezed Fe-Si height of 0.94 \r{A}, the superconducting transition at $T_{c}$ = 10 K is unusually high. In the normal state, the resistivity displays non-Fermi-liquid behavior while NMR experiments evidence weak antiferromagnetic fluctuations. According to first-principles calculations, the Fermi surface of this material is dominated by hole pockets without nesting properties, which explains the strongly suppressed tendency towards magnetic order and suggests that the emergence of superconductivity materializes in a distinct set-up, as compared to the standard $s_\pm$- and $d$-wave electron-pocket-based situations. These properties and its simple-to-implement synthesis make LaFeSiO$_{1-\delta}$ a particularly promising platform to study the interplay between structure, electron correlations and superconductivity.",2206.11690v1 2022-10-18,All-electrical spin-to-charge conversion in sputtered Bi$_x$Se$_{1-x}$,"One of the major obstacles to realizing spintronic devices such as MESO logic devices is the small signal magnitude used for magnetization readout, making it important to find materials with high spin-to-charge conversion efficiency. Although intermixing at the junction of two materials is a widely occurring phenomenon, its influence on material characterization and the estimation of spin-to-charge conversion efficiencies is easily neglected or underestimated. Here, we demonstrate all electrical spin-to-charge conversion in Bi$_x$Se$_{1-x}$ nanodevices and show how the conversion efficiency can be overestimated by tens of times depending on the adjacent metal used as a contact. We attribute this to the intermixing-induced compositional change and the properties of a polycrystal that lead to drastic changes in resistivity and spin Hall angle. Strategies to improve the spin-to-charge conversion signal in similar structures for functional devices are discussed.",2210.09792v1 2023-09-09,Intrinsic magnetic properties of the layered antiferromagnet CrSBr,"Van der Waals magnetic materials are an ideal platform to study low-dimensional magnetism. Opposed to other members of this family, the magnetic semiconductor CrSBr is highly resistant to degradation in air, which, besides its exceptional optical, electronic, and magnetic properties, is the reason the compound is receiving considerable attention at the moment. For many years, its magnetic phase diagram seemed to be well-understood. Recently, however, several groups observed a magnetic transition in magnetometry measurements at temperatures of around 40 K that is not expected from theoretical considerations, causing a debate about the intrinsic magnetic properties of the material. In this letter, we report the absence of this particular transition in magnetization measurements conducted on high-quality CrSBr crystals, attesting to the extrinsic nature of the low-temperature magnetic phase observed in other works. Our magnetometry results obtained from large bulk crystals are in very good agreement with the magnetic phase diagram of CrSBr previously predicted by the mean-field theory; A-type antiferromagnetic order is the only phase observed below the N\'eel temperature at TN = 131 K. Moreover, numerical fits based on the Curie-Weiss law confirm that strong ferromagnetic correlations are present within individual layers even at temperatures much larger than TN.",2309.04778v1 2024-01-25,Threshold displacement energy map of Frenkel pair generation in $\rm Ga_2O_3$ from machine-learning-driven molecular dynamics simulations,"$\beta$ phase gallium oxide ($\beta$-$\rm Ga_2O_3$) demonstrates tremendous potential for electronics applications and offers promising prospects for integration into future space systems with the necessity of high radiation resistance. Therefore, a comprehensive understanding of the threshold displacement energy (TDE) and the radiation-induced formation of Frenkel pairs (FPs) in this material is vital but has not yet been thoroughly studied. In this work, we performed over 5,000 molecular dynamics simulations using our machine-learning potentials to determine the TDE and investigate the formation of FPs. The average TDEs for the two Ga sites, Ga1 (tetrahedral site) and Ga2 (octahedral site), are 22.9 and 20.0 eV, respectively. While the average TDEs for the three O sites are nearly uniform, ranging from 17.0 to 17.4 eV. The generated TDE maps reveal significant differences in displacement behavior between these five atomic sites. Our developed defect identification methods successfully categorize various types of FPs in this material, with more than ten types of Ga FPs being produced during our simulations. O atoms are found to form two main types of FPs and the O split interstitial site on O1 site is most common. Finally, the recombination behavior and barriers of Ga and O FPs indicate that the O FP has a higher possibility of recovery upon annealing. Our findings provide important insights into the studies of radiation damage and defects in $\rm Ga_2O_3$ and can contribute to the design and development of $\rm Ga_2O_3$-based devices",2401.14039v2 2024-03-06,Collision Cascade-Driven Evolution of Vacancy Defects in Ni-Based Concentrated Solid-Solution Alloys,"Concentrated solid--solution alloys (CSAs) in single--phase form have recently garnered considerable attention owing to their potential for exceptional irradiation resistance. This computational study delves into the intricate interplay of alloying elements on the generation, recombination, and evolution of irradiation-induced defects. Molecular dynamics simulations were conducted for collision cascades at room temperature, spanning a range of primary knock-on atom energies from 1 to 10 keV. The investigation encompasses a series of model crystals, progressing from pure Ni to binary CSAs such as NiFe$_{20}$, NiFe, NiCr$_{20}$, and culminating in the more intricate NiFeCr$_{20}$ CSA. We observe that materials rich in chromium actively facilitate dislocation emissions and induce the nucleation of stacking fault tetrahedra in the proximity of nanovoids, owing to Shockley partial interactions. This result is validated by molecular static simulations, which calculate the surface, vacancy, and defect formation energies. Among various shapes considered, the spherical void proves to be the most stable, followed by the truncated octahedron and octahedron shapes. On the other hand, the tetrahedron cubic shape is identified as the most unstable, and stacking fault tetrahedra exhibit the highest formation energy. Notably, among the materials studied, NiCr$_{20}$ and NiFeCr$_{20}$ CSAs stood out as the sole alloys capable of manifesting this mechanism, mainly observed at high impact energies.",2403.03922v1 2024-05-08,Pressure induced metallization and loss of surface magnetism in FeSi,"Single crystalline FeSi samples with a conducting surface state (CSS) were studied under high pressure ($\textit{P}$) and magnetic field ($\textit{B}$) by means of electrical resistance ($\textit{R}$) measurements to explore how the bulk semiconducting state and the surface state are tuned by the application of pressure. We found that the energy gap ($\Delta$) associated with the semiconducting bulk phase begins to close abruptly at a critical pressure ($P_{cr}$) of ~10 GPa and the bulk material becomes metallic with no obvious sign of any emergent phases or non-Fermi liquid behavior in $\textit{R}$($\textit{T}$) in the neighborhood of $P_{cr}$ above 3 K. Moreover, the metallic phase appears to remain at near-ambient pressure upon release of the pressure. Interestingly, the hysteresis in the $\textit{R}$($\textit{T}$) curve associated with the magnetically ordered CSS decreases with pressure and vanishes at $P_{cr}$, while the slope of the $\textit{R}$($\textit{B}$) curve, d$\textit{R}$/d$\textit{B}$, which has a negative value for $\textit{P}$ < $P_{cr}$, decreases in magnitude with $\textit{P}$ and changes sign at $P_{cr}$. Thus, the CSS and the corresponding two-dimensional magnetic order collapse at $P_{cr}$ where the energy gap $\Delta$ of the bulk material starts to close abruptly, revealing the connection between the CSS and the semiconducting bulk state in FeSi.",2405.04739v1 2024-05-09,Controlled Fabrication of Native Ultra-Thin Amorphous Gallium Oxide from 2D Gallium Sulfide for Emerging Electronic Applications,"Oxidation of two-dimensional (2D) layered materials has proven advantageous in creating oxide/2D material heterostructures, opening the door for a new paradigm of low-power electronic devices. Gallium (II) sulfide ($\beta$-GaS), a hexagonal phase group III monochalcogenide, is a wide bandgap semiconductor with a bandgap exceeding 3 eV in single and few layer form. Its oxide, gallium oxide (Ga$_2$O$_3$), combines large bandgap (4.4-5.3 eV) with high dielectric constant (~10). Despite the technological potential of both materials, controlled oxidation of atomically-thin $\beta$-GaS remains under-explored. This study focuses into the controlled oxidation of $\beta$-GaS using oxygen plasma treatment, achieving ultrathin native oxide (GaS$_x$O$_y$, ~4 nm) and GaS$_x$O$_y$/GaS heterostructures where the GaS layer beneath remains intact. By integrating such structures between metal electrodes and applying electric stresses as voltage ramps or pulses, we investigate their use for resistive random-access memory (ReRAM). The ultrathin nature of the produced oxide enables low operation power with energy use as low as 0.22 nJ per operation while maintaining endurance and retention of 350 cycles and 10$^4$ s, respectively. These results show the significant potential of the oxidation-based GaS$_x$O$_y$/GaS heterostructure for electronic applications and, in particular, low-power memory devices.",2405.05632v1 2013-06-04,Constitutive Model for Material Comminuting at High Shear Rate,"The modeling of high velocity impact into brittle or quasibrittle solids is hampered by the unavailability of a constitutive model capturing the effects of material comminution into very fine particles. The present objective is to develop such a model, usable in finite element programs. The comminution at very high strain rates can dissipate a large portion of the kinetic energy of an impacting missile. The spatial derivative of the energy dissipated by comminution gives a force resisting the penetration, which is superposed on the nodal forces obtained from the static constitutive model in a finite element program. The present theory is inspired partly by Grady's model for comminution due to explosion inside a hollow sphere, and partly by analogy with turbulence. In high velocity turbulent flow, the energy dissipation rate is enhanced by the formation of micro-vortices (eddies) which dissipate energy by viscous shear stress. Similarly, here it is assumed that the energy dissipation at fast deformation of a confined solid gets enhanced by the release of kinetic energy of the motion associated with a high-rate shear strain of forming particles. For simplicity, the shape of these particles in the plane of maximum shear rate is considered to be regular hexagons. The rate of release of free energy density consisting of the sum of this energy and the fracture energy of the interface between the forming particle is minimized. The particle sizes are assumed to be distributed according to Schuhmann's power law. It is concluded that the minimum particle size is inversely proportional to the (2/3)-power of the shear strain rate, that the kinetic energy release is to proportional to the (2/3)-power, and that the dynamic comminution creates an apparent material viscosity inversely proportional to the (1/3)-power of the shear strain rate.",1306.1120v1 2005-10-03,A Study of Apparent Symmetry Breakdown in Perovskite Oxide-based Symmetric RRAM Devices,"A new model of a symmetric two-terminal non-volatile RRAM device based on Perovskite oxide thin film materials, specifically Pr1-xCaxMnO3 (PCMO), is proposed and analyzed. The model consists of two identical half-parts, which are completely characterized by the same resistance verses pulse voltage hysteresis loop, connected together in series. Even though the modeled device is physically symmetric with respect to the direction of current, it is found to exhibit switching of the resistance with the application of voltage pulses of sufficient amplitude and of different polarities. The apparent breakdown of parity conservation of the device is attributed to changes in resistance of the active material layer near the electrodes during switching. Thus the switching is history dependent, a feature that can be very useful for the construction of real non-volatile memory devices. An actual symmetric device, not previously reported in the literature and based on the proposed model, is fabricated in the PCMO material system. Measurements of the resistance of this new device generated an experimental hysteresis curve that matches well the calculated hysteresis curve of the model, thus confirming the features predicated by the new symmetric model.",0510059v1 2009-02-20,Lattice Resistance to Dislocation Motion : Singularity Distribution Approach,This paper has been withdrawn.,0902.3505v3 2015-03-03,Negative differential resistance and characteristic nonlinear electromagnetic response of a Topological Insulator,"Materials exhibiting negative differential resistance have important applications in technologies involving microwave generation, which range from motion sensing to radio astronomy. Despite their usefulness, there has been few physical mechanisms giving rise to materials with such properties, i.e. GaAs employed in the Gunn diode. In this work, we show that negative differential resistance also generically arise in Dirac ring systems, an example of which has been experimentally observed in the surface states of Topological Insulators. This novel realization of negative differential resistance is based on a completely different physical mechanism from that of the Gunn effect, relying on the characteristic non-monotonicity of the response curve that remains robust in the presence of nonzero temperature, chemical potential, mass gap and impurity scattering. As such, it opens up new possibilities for engineering applications, such as frequency upconversion devices which are highly sought for terahertz signal generation. Our results may be tested with thin films of Bi2Se3 Topological Insulators, and are expected to hold qualitatively even in the absence of a strictly linear Dirac dispersion, as will be the case in more generic samples of Bi2Se3 and other materials with topologically nontrivial Fermi sea regions.",1503.01097v4 2016-01-09,Flux trapping in superconducting accelerating cavities during cooling down with a spatial temperature gradient,"During the cool-down of a superconducting accelerating cavity, a magnetic flux is trapped as quantized vortices, which yield additional dissipation and contribute to the residual resistance. Recently, cooling down with a large spatial temperature gradient attracts much attention for successful reductions of trapped vortices. The purpose of the present paper is to propose a model to explain the observed efficient flux expulsions and the role of spatial temperature gradient during the cool-down of cavity. In the vicinity of a region with a temperature close to the critical temperature Tc,the critical fields are strongly suppressed and can be smaller than the ambient magnetic field. A region with a lower critical field smaller than the ambient field is in the vortex state. As a material is cooled down, a region with a temperature close Tc associating the vortex state domain sweeps and passes through the material. In this process, vortices contained in the vortex state domain are trapped by pinning centers that randomly distribute in the material. A number of trapped vortices can be naively estimated by using the analogy with the beam-target collision event. Based on this result, the residual resistance is evaluated. We find that a number of trapped vortices and the residual resistance are proportional to the strength of the ambient magnetic field and the inverse of the temperature gradient. The obtained residual resistance agrees well with experimental results. A material property dependence of a number of trapped vortices is also discussed.",1601.02118v2 2018-01-08,Magnetoresistance when Spin Effects on Conduction are Weak,"This paper considers certain materials, including topological insulators, where spin rotation symmetry is broken much more strongly than time reversal symmetry. When these materials are in the diffusive regime, i.e. when they have disorder that is strong enough to cause an electron to scatter many times while crossing a sample, electrons and holes move in pairs that have zero spin and are insensitive to spin physics. Working within this spinless scenario, we show that Fourier transforming the magnetoconductance with respect to external magnetic field obtains a curve describing the area distribution of loops traced by electrons and holes within the sample. We present loop area distributions of Landau levels, weak (anti)localization, conduction governed by Levy flights, and linear-in-field resistance. Of these four the last two are new results. Comparing these distributions, we argue that the linear-in-field resistance seen in some topological insulators is caused by the same diffusive scattering that causes weak antilocalization. The difference is that linear-in-field resistance materials retain a level of quantum coherence that is usually seen only on the surface of 2-D wires or in ring geometries. In an appendix we include some speculative material about linear-in-temperature resistance.",1801.02663v6 2020-09-04,Thermal conductivity of PbTe-CoSb3 bulk polycrystalline composite: the role of microstructure and interface thermal resistance,"Systematic experimental and theoretical research on the role of microstructure and interface thermal resistance on the thermal conductivity of the PbTe-CoSb3 bulk polycrystalline composite is presented. In particular, the correlation between the particle size of the dispersed phase and interface thermal resistance (R_{int}) on the phonon thermal conductivity (\kappa_{ph}) is discussed. With this aim, a series of PbTe-CoSb_3 polycrystalline composite materials with the different particle sizes of CoSb_3 was prepared. The structural (XRD) and microstructural analysis (SEM/EDXS) confirmed assumed chemical and phase compositions. The acoustic impedance difference (\Delta Z) was determined from measured sound velocities in PbTe and CoSb_3 phases. The interface thermal resistance (R_{int}) was calculated using the Debye model and agrees with the experimental R_{int}. It is shown that the \kappa_{ph} of the composite may be reduced when the particle size of the dispersed phase (CoSb_3) is smaller than the critical value of ~230nm. This relationship was concluded to be crucial for controlling the heat transport phenomena in composite thermoelectric materials. The selection of the components with different elastic properties (acoustic impedance) and particle size smaller than the Kapitza radius leads to a new direction in the engineering of composite TE materials with designed thermal properties",2009.02190v2 2020-09-20,"Development of a computational software in Python, used to study the materials resistance in beams","In this research, we do a software writing in Python to calculate the efforts, bending moments and deformations in beams of different materials. This computational tool, that we developed, is of great help in area of computational physical, more exactly in resistance of materials, which serves as support for researchers and teachers especially in physics and civil engineering, of the part of statics, who wish to carry out the modeling of the functions, involved in the calculation of resistance in beams in a practical and simple way, using the software presented in this article. In order to carry out this software, we are going to use the following methods: the double-integration method and the conjugate-beam method, which will serve as the basis of calculation to find the mathematical expressions involved in the analysis of resistance in beams, then we will perform the implementation of the aforementioned methods, using Python as the programming language. As a final step in this project, the graphical interface of said calculation tool will be made using the Python 3.0 Tkinter library. In this work, we show the results of the graphs of the stress profiles, bending moments and deformations, for the case of different types of beams, load and force distributions applied to them. Where we were also able to conclude that a calculation software was successfully built, dedicated to the analysis of efforts and deformations in beams made of different materials.",2009.09448v2 2022-07-01,High-throughput analysis of Fröhlich-type polaron models,"The electronic structure of condensed matter can be significantly affected by the electron-phonon interaction, leading to important phenomena such as electrical resistance, superconductivity or the formation of polarons. This interaction is often neglected in band structure calculations but can have a strong impact on band gaps or optical spectra. Commonly used frameworks for electron-phonon energy corrections are the Allen-Heine-Cardona theory and the Fr\""ohlich model. While the latter shows qualitative agreement with experiment for many polar materials, its simplicity should bring hard limits to its applicability in real materials. Improvements can be made by introducing a generalized version of the model, which considers anisotropic and degenerate electronic bands, and multiple phonon branches. In this work, we search for trends and outliers on over a thousand materials in existing databases of phonon and electron band structures. We use our results to identify the limits of applicability of the standard Fr\""olich model by comparing to the generalized version, and by testing its basic hypothesis of a large radius for the polaronic wavefunction and the corresponding atomic displacement cloud. Among our extended set of materials, most exhibit large polaron behavior as well as validity of the perturbative treatment. For the valence band, there is also a significant fraction of the materials for which the perturbative treatment cannot be applied and/or for which the size of the self-trapping region is close to the atomic repetition distance. We find a large variety of behaviors, and employ much more accurate, fully ab initio Allen-Heine-Cardona calculations to understand extreme cases, where the Fr\""ohlich model should fail and unusually large zero-point renormalization energies occur.",2207.00364v1 2013-03-26,Molecular Memory with Atomically-Smooth Graphene Contacts,"We report the use of bilayer graphene as an atomically-smooth contact for nanoscale devices. A two-terminal Bucky ball (C60) based molecular memory is fabricated with bilayer graphene as a contact on the polycrystalline nickel electrode. Graphene provides an atomically-smooth covering over an otherwise rough metal surface. The use of graphene additionally prohibits the electromigration of nickel atoms into the C60 layer. The devices exhibit a low-resistance state in the first sweep cycle and irreversibly switch to a high resistance state at 0.8-1.2 V bias. The reverse sweep has a hysteresis behavior as well. In the subsequent cycles, the devices retain the high-resistance state, thus making it write-once read-many memory (WORM). The ratio of current in low-resistance to high-resistance state is lying in 20-40 range for various devices with excellent retention characteristics. Control sample without the bilayer graphene shows random hysteresis and switching.",1303.6603v1 2020-04-10,Vortex Dynamics and Dissipation Under High-amplitude Microwave Drive,"In this paper, we describe the vortex dynamics under high-amplitude microwave drive and its effect on the surface resistance of superconductors. The vortex surface resistance is calculated with a Montecarlo approach, where the vortex motion equation is solved for a collection of vortex flux lines each oscillating within a random pinning landscape. This approach is capable of providing a detailed description of the microscopic vortex dynamics and in turn important insights into the microwave field amplitude dependence of the vortex surface resistance. The numerical simulations are compared against experimental data of vortex surface resistance at high microwave amplitude measured by means of bulk niobium superconducting-radio frequency cavities operating at 1.3 GHz. The good qualitative agreement of simulations and experiments suggests that the non-linear dependence of the trapped flux surface resistance with the microwave field amplitude is generated by progressive microwave depinning and vortex jumps.",2004.05083v2 2015-07-17,Resistive thrust production can be as crucial as added mass mechanisms for inertial undulatory swimmers,"In this paper, we address a crucial point regarding the description of moderate to high Reynolds numbers aquatic swimmers. For decades, swimming animals have been classified in two different families of propulsive mechanisms based on the Reynolds number: the ""resistive"" swimmers, using local friction to produce the necessary thrust force for locomotion at low Reynolds number and the ""reactive"" swimmers, lying in the high Reynolds range, and using added mass acceleration (described by perfect fluid theory). However, inertial swimmers are also systems that dissipate energy, due to their finite size, therefore involving strong resistive contributions, even for high Reynolds numbers. Using a complete model for the hydrodynamic forces, involving both reactive and resistive contributions, we revisit here the physical mechanisms responsible for the thrust production of such swimmers. We show, for instance, that the resistive part of the force balance is as crucial as added mass effects in the modeling of the thrust force, especially for elongated species. The conclusions brought by this work may have significant contributions to the understanding of complex swimming mechanisms, especially for the future design of artificial swimmers.",1507.04952v1 2022-07-13,Memristive and tunneling effects in 3D interconnected silver nanowires,"Due to their memristive properties nanowire networks are very promising for neuromorphic computing applications. Indeed, the resistance of such systems can evolve with the input voltage or current as it confers a synaptic behaviour to the device. Here, we propose a network of silver nanowires (Ag-NWs) which are grown in a nanopourous membrane with interconnected nanopores by electrodeposition. This bottom-up approach fabrication method gives a conducting network with a 3D architecture and a high density of Ag-NWs. The resulting 3D interconnected Ag-NW network exhibits a high initial resistance as well as a memristive behavior. It is expected to arise from the creation and the destruction of conducting silver filaments inside the Ag-NW network. Moreover, after several cycles of measurement, the resistance of the network switches from a high resistance regime, in the GOhm range, with a tunnel conduction to a low resistance regime, in the kOhm range.",2207.06338v1 2011-05-06,Giant microwave photoresistivity in a high-mobility quantum Hall system,"We report the observation of a remarkably strong microwave photoresistivity effect in a high-mobility two-dimensional electron system subject to a weak magnetic field and low temperature. The effect manifests itself as a giant microwave-induced resistivity peak which, in contrast to microwave-induced resistance oscillations, appears only near the second harmonic of the cyclotron resonance and only at sufficiently high microwave frequencies. Appearing in the regime linear in microwave intensity, the peak can be more than an order of magnitude stronger than the microwave-induced resistance oscillations and cannot be explained by existing theories.",1105.1390v1 2014-11-19,Towards pristine graphene-metal interface and microstructures: Laser assisted direct patterning on Epitaxial graphene,"Graphene-metal contact resistance is governed by both intrinsic and extrinsic factors. Intrinsically, both the density of states bottleneck near the Dirac point and carrier reflection at the graphene-metal interface lead to a high contact resistance. Moreover, graphene exhibits insulating behavior for out-of-the-plane conduction. Extrinsically, surface contamination introduced by photoresist residue or different adsorbed species during standard lithography processing alters graphene's intrinsic properties by uncontrolled doping and increased scattering which results in high and inconsistent contact resistance. Here we demonstrate a femto-second laser assisted direct patterning of graphene microstructures that enables us to study both intrinsic and extrinsic effects on the graphene-metal interface. We show that a clean graphene-metal interface is not sufficient to obtain contact resistance approaching the intrinsic limit set by the quantum resistance. We also demonstrated that unlike CVD graphene, edge state conduction (or end-contact) is not spontaneously formed by metal deposition in case of graphene grown on SiC(0001). We conclude that for epitaxial graphene, intentional end-contact formation is necessary to obtain contact resistance near the quantum contact resistance limit.",1411.5114v1 2023-11-08,An attention-based deep learning network for predicting Platinum resistance in ovarian cancer,"Background: Ovarian cancer is among the three most frequent gynecologic cancers globally. High-grade serous ovarian cancer (HGSOC) is the most common and aggressive histological type. Guided treatment for HGSOC typically involves platinum-based combination chemotherapy, necessitating an assessment of whether the patient is platinum-resistant. The purpose of this study is to propose a deep learning-based method to determine whether a patient is platinum-resistant using multimodal positron emission tomography/computed tomography (PET/CT) images. Methods: 289 patients with HGSOC were included in this study. An end-to-end SE-SPP-DenseNet model was built by adding Squeeze-Excitation Block (SE Block) and Spatial Pyramid Pooling Layer (SPPLayer) to Dense Convolutional Network (DenseNet). Multimodal data from PET/CT images of the regions of interest (ROI) were used to predict platinum resistance in patients. Results: Through five-fold cross-validation, SE-SPP-DenseNet achieved a high accuracy rate and an area under the curve (AUC) in predicting platinum resistance in patients, which were 92.6% and 0.93, respectively. The importance of incorporating SE Block and SPPLayer into the deep learning model, and considering multimodal data was substantiated by carrying out ablation studies and experiments with single modality data. Conclusions: The obtained classification results indicate that our proposed deep learning framework performs better in predicting platinum resistance in patients, which can help gynecologists make better treatment decisions. Keywords: PET/CT, CNN, SE Block, SPP Layer, Platinum resistance, Ovarian cancer",2311.04769v1 2000-08-17,Development of Gold Contacted Flip-chip Detectors with IMARAD CZT,"We present initial results from our evaluation of a gold-contacted pixellated detector using cadmium zinc telluride substrate produced by IMARAD Imaging Systems. The Horizontal Bridgman (HB) grown crystals from IMARAD have been shown to produce high resolution photopeaks, but they are also seen to have large leakage current. Our previous tests with IMARAD CZT showed that the use of indium anodes and gold cathode improved the resistivity compared to the standard indium-contacted detectors. We seek to test whether simple evaporated gold contacts alone could also reduce the leakage current and thus improve the spectral resolution, especially in the 10-100 keV energy range. We have fabricated several metal-semiconductor-metal (MSM) detectors with a 4x4 array of pixels on 10x10 mm substrates. Measurements of the detectors' leakage current, spectral response, and temperature sensitivity are presented and compared to IMARAD's ohmic contact detector and gold contact MSM detectors made of High Pressure Bridgman (HPB) material. Finally, we show preliminary results from a tiled flip-chip pixellated detector made using the IMARAD detectors.",0008275v1 1997-09-21,Microwave properties of $(Pr_xY_{1-x})Ba_2Cu_3O_{7-δ}$ : Influence of magnetic scattering,"We report measurements of the surface impedance $Z_s=R_s+iX_s$ of $(Pr_xY_{1-x})Ba_2Cu_3O_{7-\delta}$, $(x=0,0.15,0.23,0.3,0.4,0.5)$. Increasing $Pr$ concentration leads to some striking results not observed in samples doped by non-magnetic constituents. The three principal features of the $R_s(T)$ data - multiple structure in the transition, a high residual resistance and, at high $Pr$ concentrations, an upturn of the low $T$ data, are all characteristic of the influence of magnetic scattering on superconductivity, and appear to be common to materials where magnetism and superconductivity coexist. The low $T$ behavior of $\lambda (T)$ appears to change from $T$ to $T^4$ at large $Pr$ doping, and provides evidence of the influence of magnetic pairbreaking of the $Pr$.",9709232v1 1997-12-08,High frequency magneto-electrodynamics of La_(1-x)Sr_xMnO3 single crystals,"The radio frequency (RF) response of La1-xSrxMnO3 single crystals reveal a variety of features associated with the structural, electronic and magnetic properties of the system. The resonance technique operating at ~ 4 MHz employed in this study is sensitive to small changes in both the magnetic susceptibility and resistivity of the samples. Very sharp changes in frequency are observed at the ferromagnetic (FM) and structural phase transitions in both the metallic (x = 0.175) and insulating (0.125) crystals studied. In addition to the known transitions identified as FM and orthorhombic distortions, our experiments show rich structures which are not observed in conventional DC magnetization and transport experiments. Our results demonstrate that RF experiments are ideally suited to investigate the complex phase diagram in the manganites. The colossal frequency change that we observe at the FM transition in the La1-xSrxMnO3 crystals is indicative of the enormous potential for using these materials in high frequency switching applications.",9712093v1 1999-04-28,Structure and properties of a novel fulleride Sm6C60,"A novel fulleride Sm6C60 has been synthesized using high temperature solid state reaction. The Rietveld refinement on high resolution synchrotron X-ray powder diffraction data shows that Sm6C60 is isostructural with body-centered cubic A6C60 (A=K, Ba). Raman spectrum of Sm6C60 is similar to that of Ba6C60, and the frequencies of two Ag modes in Sm6C60 are nearly the same as that of Ba6C60, suggesting that Sm is divalent and hybridization between C60 molecules and the Sm atom could exist in Sm6C60. Resistivity measurement shows a weak T-linear behavior above 180 K, the transport at low temperature is mainly dominated by granular-metal theory.",9904404v1 2000-04-10,Magnetotransport study of the charged stripes in high-T_c cuprates,"We present a study of the in-plane and out-of-plane magnetoresistance (MR) in heavily-underdoped, antiferromagnetic YBa_{2}Cu_{3}O_{6+x}, which reveals a variety of striking features. The in-plane MR demonstrates a ""d-wave""-like anisotropy upon rotating the magnetic field H within the ab plane. With decreasing temperature below 20-25 K, the system acquires memory: exposing a crystal to the magnetic field results in a persistent in-plane resistivity anisotropy. The overall features can be explained by assuming that the CuO_2 planes contain a developed array of stripes accommodating the doped holes, and that the MR is associated with the field-induced topological ordering of the stripes.",0004135v1 2000-07-11,Grain boundary effects on magnetotransport in bi-epitaxial films of La$_{0.7}$Sr$_{0.3}$MnO$_3$,"The low field magnetotransport of La$_{0.7}$Sr$_{0.3}$MnO$_3$ (LSMO) films grown on SrTiO$_3$ substrates has been investigated. A high qualtity LSMO film exhibits anisotropic magnetoresistance (AMR) and a peak in the magnetoresistance close to the Curie temperature of LSMO. Bi-epitaxial films prepared using a seed layer of MgO and a buffer layer of CeO$_2$ display a resistance dominated by grain boundaries. One film was prepared with seed and buffer layers intact, while a second sample was prepared as a 2D square array of grain boundaries. These films exhibit i) a low temperature tail in the low field magnetoresistance; ii) a magnetoconductance with a constant high field slope; and iii) a comparably large AMR effect. A model based on a two-step tunneling process, including spin-flip tunneling, is discussed and shown to be consistent with the experimental findings of the bi-epitaxial films.",0007194v1 2001-02-23,Temperature Dependence of Low-Lying Electronic Excitations of LaMnO_3,"We report on the optical properties of undoped single crystal LaMnO_3, the parent compound of the colossal magneto-resistive manganites. Near-Normal incidence reflectance measurements are reported in the frequency range of 20-50,000 cm-1 and in the temperature range 10-300 K. The optical conductivity, s_1(w), is derived by performing a Kramers-Kronig analysis of the reflectance data. The far-infrared spectrum of s_1(w) displays the infrared active optical phonons. We observe a shift of several of the phonon to high frequencies as the temperature is lowered through the Neel temperature of the sample (T_N = 137 K). The high-frequency s_1(w) is characterized by the onset of absorption near 1.5 eV. This energy has been identified as the threshold for optical transitions across the Jahn-Teller split e_g levels. The spectral weight of this feature increases in the low-temperature state. This implies a transfer of spectral weight from the UV to the visible associated with the paramagnetic to antiferromagnetic state. We discuss the results in terms of the double exchange processes that affect the optical processes in this magnetic material.",0102437v1 2001-02-27,Anisotropic three-dimentional magnetic fluctuations in heavy fermion CeRhIn5,"CeRhIn5 is a heavy fermion antiferromagnet that orders at 3.8 K. The observation of pressure-induced superconductivity in CeRhIn5 at a very high Tc of 2.1 K for heavy fermion materials has led to speculations regarding to its magnetic fluctuation spectrum. Using magnetic neutron scattering, we report anisotropic three-dimensional antiferromagnetic fluctuations with an energy scale of less than 1.7 meV for temperatures as high as 3Tc. In addition, the effect of the magnetic fluctuations on electrical resistivity is well described by the Born approximation.",0102503v1 2001-12-21,First order transition from ferromagnetism to antiferromagnetism in Ce(Fe$_{0.96}$Al$_{0.04}$)$_2$: a magnetotransport study,"The magnetotransport behaviour is investigated in detail across the first order magnetic phase transition from ferromagnetic to antiferromagnetic state in polycrystalline Ce(Fe$_{0.96}$Al$_{0.04}$)$_2$ sample. The study clearly brings out various generic features associated with a first order transition, viz., hysteresis, phase coexistence, supercooling and superheating, presence and limits of the metastable regimes. These results of magnetotransport study exhibit and support all the interesting thermomagnetic history effects that were observed in our earlier dc-magnetisation study on the same sample. Most notable here is the initial (or virgin) resistivity vs. field curve lying outside the hysteretic ""butterfly shaped"" magnetoresistivity loops obtained on cyclying the magnetic field between high enough positive and negative strengths. These findings, bearing one-to-one similarity with the data obtained in their magnetic counterpart (i.e., dc-magnetisation), have been ascribed an origin due to the arresting of this first order transition kinetics at low temperature and high magnetic field.",0112408v1 2002-08-07,Transport critical current densities and n factors in mono- and multifilamentary MgB2/Fe tapes and wires using fine powders,"Mono- and multifilamentary MgB2/Fe tapes and wires with high transport critical current densities have been prepared using the powder-in-tube (PIT) process. The fabrication details are described. The effect of powder grain sizes and recrystallization temperature on jc has been investigated. At 25K and 1 T, jc values close to 105 A/cm2 were measured, while jc of 106 A/cm2 were extrapolated for 4.2K/0T in our monofilamentary tape. MgB2/Fe tapes exhibit high exponential n factors for the resistive transition: n ~ 80 and 40 were found at 5 T and 7 T, respectively. The highest transport jc values obtained so far in MgB2/Fe wires with 7 filaments were 1.1 * 105 A/cm2 at 4.2 K and in a field of 2 T, which is still lower than for monofilamentary tapes. Improved deformation and recovering processing is expected to lead to higher jc values.",0208133v1 2004-02-20,Metal-insulator transition and glassy behavior in two-dimensional electron systems,"Studies of low-frequency resistance noise demonstrate that glassy freezing occurs in a two-dimensional electron system in silicon in the vicinity of the metal-insulator transition (MIT). The width of the metallic glass phase, which separates the 2D metal and the (glassy) insulator, depends strongly on disorder, becoming extremely small in high-mobility (low-disorder) samples. The glass transition is manifested by a sudden and dramatic slowing down of the electron dynamics, and by a very abrupt change to the sort of statistics characteristic of complicated multistate systems. In particular, the behavior of the second spectrum, an important fourth-order noise statistic, indicates the presence of long-range correlations between fluctuators in the glassy phase, consistent with the hierarchical picture of glassy dynamics.",0402535v1 2004-04-21,Formation and Thermal Stability of sub-10 nm Carbon Templates on Si(100),"We report a lithographic process for creating high-resolution (<10 nm) carbon templates on Si(100). A scanning electron microscope, operating under low vacuum (10E-6 mbar), produces a carbon-containing deposit (""contamination resist"") on the silicon surface via electron-stimulated dissociation of ambient hydrocarbons, water and other adsorbed molecules. Subsequent annealing at temperatures up to 1320 K in ultra-high vacuum removes SiO2 and other contaminants, with no observable change in dot shape. The annealed structures are compatible with subsequent growth of semiconductors and complex oxides. Carbon dots with diameter as low as 3.5 nm are obtained with a 200 us electron-beam exposure time.",0404505v1 2005-04-19,High temperature magnetic ordering in La2RuO5,"Magnetic susceptibility, heat capacity and electrical resistivity measurements have been carried out on a new ruthenate, La2RuO5 (monoclinic, space group P21/c) which reveal that this compound is a magnetic semiconductor with a high magnetic ordering temperature of 170K. The entropy associated with the magnetic transition is 8.3 J/mole-K -close to that expected for the low spin (S=1) state of Ru4+ ions. The low temperatures specific heat coefficient g is found to be nearly zero consistent with the semiconducting nature of the compound. The magnetic ordering temperature of La2RuO5 is comparable to the highest known Curie temperature of another ruthenate, namely, metallic SrRuO3, and in both these compounds the nominal charge state of Ru is 4+.",0504489v1 2006-05-11,Multifilament YBa2Cu3O6+x -coated conductors with minimized coupling losses,"We report an experimental approach to making multifilament coated conductors with low losses in applied time-varying magnetic field. Previously, the multifilament conductors obtained for that purpose by laser ablation suffered from high coupling losses. Here we report how this problem can be solved. When the substrate metal in the grooves segregating the filaments is exposed to oxygen, it forms high resistivity oxides that electrically insulate the stripes from each other and from the substrate. As the result, the coupling loss has become negligible over the entire range of tested parameters (magnetic field amplitudes B and frequencies f) available to us.",0605313v1 2006-06-17,The thermally activated motion of vortex bundles and the anomalous Hall effect in type-II conventional and high-Tc superconductors,"The anomalous Hall effect in type-II conventional and high-Tc superconductors is investigated based on the proposed novel theory of the thermally activated motion of vortex bundles over a directional-dependent energy barrier. Our calculations demonstrate clearly that anomalous Hall effect is induced by the competition between the Magnus force and the random collective pinning force of the vortex bundle. The Hall as well as the longitudinal resistivity for constant temperature and constant applied magnetic field of type-II superconducting films and bulk materials are calculated. The reentry phenomenon is also investigated. All the results are in good agreement with the experiments.",0606464v2 1999-11-30,Analysis of trap spectra in LEC and epitaxial GaAs,"Different methods of trap parameter measurement are analysed. Transient photoconductivity and thermally stimulated effects were used to investigate the influence of traps in LEC SI-GaAs and high resistivity epitaxial GaAs. The peculiarities of the TSC were analysed and shown to be related to the influence of crystal micro-inhomogeneities.",9911048v1 2006-08-25,The Effects of Preheating of a Fine Tungsten Wire and the Polarity of a High-Voltage Electrode on the Energy Characteristics of an Electrically Exploded Wire in Vacuum,"Results obtained from experimental and numerical studies of tungsten wires electrical explosion in vacuum are presented. The experiments were performed both with and without preheating of the wires, using positive or negative polarity of a high-voltage electrode. Preheating is shown to increase energy deposition in the wire core due to a longer resistive heating stage. The effect was observed both in single wire and wire array experiments. The evolution of the phase state of the wire material during explosion was examined by means of one-dimensional numerical simulation using a semiempirical wide-range equation of state describing the properties of tungsten with allowance made for melting and vaporization.",0608251v1 2007-03-11,A low-noise ferrite magnetic shield,"Ferrite materials provide magnetic shielding performance similar to commonly used high permeability metals but have lower intrinsic magnetic noise generated by thermal Johnson currents due to their high electrical resistivity. Measurements inside a ferrite shield with a spin-exchange relaxation-free atomic magnetometer reveal a noise level of 0.75 fT Hz^(-1/2), 25 times lower than what would be expected in a comparable mu-metal shield. The authors identify a 1/f component of the magnetic noise due to magnetization fluctuations and derive general relationships for the Johnson current noise and magnetization noise in cylindrical ferromagnetic shields in terms of their conductivity and complex magnetic permeability.",0703115v2 2007-08-14,The zero-energy state in graphene in a high magnetic field,"The fate of the charge-neutral Dirac point in graphene in a high magnetic field $H$ has been investigated at low temperatures ($T\sim$ 0.3 K). In samples with small $V_0$ (the gate voltage needed to access the Dirac point), the resistance $R_0$ at the Dirac point diverges steeply with $H$, signalling a crossover to an insulating state in intense field. The approach to the insulating state is highly unusual. Despite the steep divergence in $R_0$, the profile of $R_0$ vs. $T$ in fixed $H$ saturates to a $T$-independent value below 2 K, consistent with charge carrying gapless excitations.",0708.1959v2 2008-03-25,Superconductivity at 43 K in Samarium-arsenide Oxides $SmFeAsO_{1-x}F_x$,"Since the discovery of high-transition temperature ($T_c$) superconductivity in layered copper oxides, extensive efforts have been devoted to explore the higher $T_c$ superconductivity. However, the $T_c$ higher than 40 K can be obtained only in the copper oxide superconductors so far. The highest reported value of $T_c$ for non-copper-oxide bulk superconductivity is 39 K in $MgB_2$.\cite{jun} The $T_c$ of about 40 K is close to or above the theoretical value predicted from BCS theory.\cite{mcmillan} Therefore, it is very significant to search for non-copper oxide superconductor with the transition temperature higher than 40 K to understand the mechanism of high-$T_c$ superconductivity. Here we report the discovery of bulk superconductivity in samarium-arsenide oxides $SmFeAsO_{1-x}F_x$ with ZrCuAiAs type structure. Resistivity and magnetization measurements show strong evidences for transition temperature as high as 43 K. $SmFeAsO_{1-x}F_x$ is the first non-copper oxide superconductor with $T_c$ higher than 40 K. The $T_c$ higher than 40 K may be a strong argument to consider $SmFeAsO_{1-x}F_x$ as an unconventional superconductor.",0803.3603v2 2008-04-21,CeFePO: A Heavy Fermion Metal with Ferromagnetic Correlations,"The ground state properties of CeFePO, a homologue of the new high temperature superconductors RFePnO(1-x)Fx, were studied by means of susceptibility, specific heat, resistivity, and NMR measurements on polycrystals. All the results demonstrate that this compound is a magnetically non-ordered heavy Fermion metal with a Kondo temperature TK~10K, a Sommerfeld coefficient gamma=700mJ/molK2 and a mass enhancement factor of the order of 200. The absence of a Fe-contribution to the effective moment at high temperatures indicates that the magnetism in CeFePO is completely dominated by the effect of Ce. Thus the strong electronic correlation effects originate from the Ce-4f electrons rather than from the Fe-3d electrons. An enhanced Sommerfeld-Wilson ratio R=5.5 as well as a Korringa product S0/T1TK2~0.065 well below 1 indicate the presence of ferromagnetic correlations. Therefore, CeFePO appears to be on the non-magnetic side of a ferromagnetic instability.",0804.3250v2 2008-07-05,"Growth and characterization of A_{1-x}K_xFe_2As_2 (A = Ba, Sr) single crystals with x=0 - 0.4","Single crystals of A$_{1-x}$K$_x$Fe$_2$As$_2$ (A=Ba, Sr) with high quality have been grown successfully by FeAs self-flux method. The samples have sizes up to 4 mm with flat and shiny surfaces. The X-ray diffraction patterns suggest that they have high crystalline quality and c-axis orientation. The non-superconducting crystals show a spin-density-wave (SDW) instability at about 173 K and 135 K for Sr-based and Ba-based compound, respectively. After doping K as the hole dopant into the BaFe$_2$As$_2$ system, the SDW transition is smeared, and superconducting samples with the compound of Ba$_{1-x}$K$_x$Fe$_2$As$_2$ (0 $< x \leqslant$ 0.4) are obtained. The superconductors characterized by AC susceptibility and resistivity measurements exhibit very sharp superconducting transition at about 36 K, 32 K, 27 K and 23 K for x= 0.40,0.28,0.25 and 0.23, respectively.",0807.0759v3 2008-08-18,A Ni-based Superconductor: the Heusler Compound ZrNi$_2$Ga,"This work reports on the novel Heusler superconductor ZrNi2Ga. Compared to other nickel-based superconductors with Heusler structure, ZrNi2Ga exhibits a relatively high superconducting transition temperature of Tc=2.9 K and an upper critical field of 1.5 T. Electronic structure calculations show that this relatively high transition temperature is caused by a van Hove singularity, which leads to an enhanced density of states at the Fermi energy. The van Hove singularity originates from a higher order valence instability at the L-point in the electronic structure. The enhanced density of states at the Fermi level was confirmed by specific heat and susceptibility measurements. Although many Heusler compounds are ferromagnetic, our measurements of ZrNi2Ga indicate a paramagnetic state above Tc and could not reveal any traces of magnetic order down to temperatures of at least 0.35 K. We investigated in detail the superconducting state with specific heat, magnetization, and resistivity measurements. The resulting data show the typical behavior of a conventional, weakly coupled BCS (s-wave) superconductor.",0808.2356v1 2008-10-03,"Small anisotropy, weak thermal fluctuations, and high field superconductivity in Co-doped iron pnictide Ba(Fe1-xCox)2As2","We performed high-field magnetotransport and magnetization measurements on a single crystal of the 122-phase iron pnictide Ba(Fe1-xCox)2As2. Unlike the HTS cuprates and 1111-phase oxypnictides, Ba(Fe1-xCox)2As2 showed practically no broadening of the resistive transitions under magnetic fields up to 45 T. The mass anisotropy gamma = Hc2ab/Hc2c deduced from the slopes of the upper critical field dHc2ab/dT = 4.9T/K and dHc2c/dT = 2.5T/K decreases from ~2 near Tc, to ~1.5 at lower temperatures. We observed the irreversibility field close to Hc2, and a rather unusual symmetric volume pinning force curve Fp(H) suggestive of strong pinning nano-structure.",0810.0699v2 2009-05-01,Highly segmented thin microstrip detector with data-driven fast readout,"In September 2008 the Slim5 collaboration submitted a low material budget silicon demonstrator to test with 12 GeV/c protons, at the PS-T9 test-beam at CERN. Inside the reference telescope, two different detectors were placed as device under test (DUT). The first was a 4k-Pixel Matrix of Deep N Well MAPS, developed in a 130 nm CMOS Technology, providing digital sparsified readout. The other one was a high resistivity double sided silicon detector, with short strips at 45-degree angle to the detector's edge, read out by the FSSR2 chip. The FSSR2 is a 128 channel data-driven fast readout chip developed by Fermilab and INFN. In this paper we describe the main features of latter sensor, the striplet. The primary goal of the test was to measure the efficiency and the resolution of the striplets. The data-driven approach of the FSSR2 readout chips has been fully exploited by the DAQ system.",0905.0083v3 2009-10-08,Structural and transport properties of Sr2VO{3-delta}FeAs superconductors with different oxygen deficiencies,"Sr2VO{3-delta}FeAs superconductors with different oxygen deficiencies have been successfully fabricated. It is found that the superconducting transition temperature drops down monotonically with the increase of oxygen deficiency. The diminishing of superconductivity is accompanied by the enhancement of residual resistivity, indicating an unraveled scattering effect induced by the oxygen deficiency. The highest superconducting transition temperature at about 40 K is achieved near the stoichiometrical sample Sr$_2$VO$_{3}$FeAs. Surprisingly, the X-ray photoelectron spectroscopy (XPS) shows that the vanadium has a ""5+"" valence state in the samples. The Hall effect measurements reveal that the density of charge carriers (electron-like here) varies qualitatively with the increase of oxygen deficiency. Magnetotransport measurements show that the superconducting transition changes from one-step-like shape at low fields to two-step-like one at high fields, indicating a high anisotropy.",0910.1537v2 2010-04-22,Optimizing Transistor Performance of Percolating Carbon Nanotube Networks,"In percolating networks of mixed metallic and semiconducting CNTs, there is a tradeoff between high on-current (dense networks) and high on/off ratio (sparse networks in which the metallic CNT fraction is not percolating). Experiments on devices in a transistor configuration and Monte Carlo simulations were performed to determine the scaling behavior of device resistivity as a function of channel length (L) for CNT density p in the range 0.04 - 1.29 CNT/{\mu}m^2 in the on- and off-states. Optimized devices with field-effect mobility up to 50 cm^2/Vs at on/off ratio > 10^3 were obtained at W = 50 {\mu}m, L > 70 {\mu}m for p = 0.54 - 0.81 CNTs/{\mu}m^2.",1004.4009v1 2010-06-25,Spin and charge dynamics in [TbPc$_2$]$^0$ and [DyPc$_2$]$^0$ single molecule magnets,"Magnetization, AC susceptibility and $\mu$SR measurements have been performed in neutral phthalocyaninato lanthanide ([LnPc$_2]^0$) single molecule magnets in order to determine the low-energy levels structure and to compare the low-frequency spin excitations probed by means of macroscopic techniques, such as AC susceptibility, with the ones explored by means of techniques of microscopic character, such as $\mu$SR. Both techniques show a high temperature thermally activated regime for the spin dynamics and a low temperature tunneling one. While in the activated regime the correlation times for the spin fluctuations estimated by AC susceptibility and $\mu$SR basically agree, clear discrepancies are found in the tunneling regime. In particular, $\mu$SR probes a faster dynamics with respect to AC susceptibility. It is argued that the tunneling dynamics probed by $\mu$SR involves fluctuations which do not yield a net change in the macroscopic magnetization probed by AC susceptibiliy. Finally resistivity measurements in [TbPc$_2]^0$ crystals show a high temperature nearly metallic behaviour and a low temperature activated behaviour.",1006.4919v1 2010-09-17,Graphene Transport at High Carrier Densities using a Polymer Electrolyte Gate,"We report the study of graphene devices in Hall-bar geometry, gated with a polymer electrolyte. High densities of 6 $\times 10^{13}/cm^{2}$ are consistently reached, significantly higher than with conventional back-gating. The mobility follows an inverse dependence on density, which can be correlated to a dominant scattering from weak scatterers. Furthermore, our measurements show a Bloch-Gr\""uneisen regime until 100 K (at 6.2 $\times10^{13}/cm^{2}$), consistent with an increase of the density. Ubiquitous in our experiments is a small upturn in resistivity around 3 $\times10^{13}/cm^{2}$, whose origin is discussed. We identify two potential causes for the upturn: the renormalization of Fermi velocity and an electrochemically-enhanced scattering rate.",1009.3367v2 2010-10-28,Poole-Frenkel Effect and Phonon-Assisted Tunneling in GaAs Nanowires,"We present electronic transport measurements of GaAs nanowires grown by catalyst-free metal-organic chemical vapor deposition. Despite the nanowires being doped with a relatively high concentration of substitutional impurities, we find them inordinately resistive. By measuring sufficiently high aspect-ratio nanowires individually in situ, we decouple the role of the contacts and show that this semi-insulating electrical behavior is the result of trap-mediated carrier transport. We observe Poole-Frenkel transport that crosses over to phonon-assisted tunneling at higher fields, with a tunneling time found to depend predominantly on fundamental physical constants as predicted by theory. By using in situ electron beam irradiation of individual nanowires we probe the nanowire electronic transport when free carriers are made available, thus revealing the nature of the contacts.",1010.6086v1 2010-11-23,NaIrO3 - A pentavalent post-perovskite,"Sodium iridium(V) oxide, NaIrO3, was synthesized by a high pressure solid state method and recovered to ambient conditions. It is found to be isostructural with CaIrO3, the much-studied structural analogue of the high-pressure post-perovskite phase of MgSiO3. Among the oxide post-perovskites, NaIrO3 is the first example with a pentavalent cation. The structure consists of layers of corner- and edge-sharing IrO6 octahedra separated by layers of NaO8 bicapped trigonal prisms. NaIrO3 shows no magnetic ordering and resistivity measurements show non-metallic behavior. The crystal structure, electrical and magnetic properties are discussed and compared to known post-perovskites and pentavalent perovskite metal oxides.",1011.5125v2 2010-12-11,Transport Spin Polarization of High-Curie Temperature MnBi Films,"We report on the study of the structural, magnetic and transport properties of highly textured MnBi films with the Curie temperature of 628K. In addition to detailed measurements of resistivity and magnetization, we measure transport spin polarization of MnBi by Andreev reflection spectroscopy and perform fully relativistic band structure calculations of MnBi. A spin polarization from 51\pm1 to 63\pm1% is observed, consistent with the calculations and with an observation of a large magnetoresistance in MnBi contacts. The band structure calculations indicate that, in spite of almost identical densities of states at the Fermi energy, the large disparity in the Fermi velocities leads to high transport spin polarization of MnBi. The correlation between the values of magnetization and spin polarization is discussed.",1012.2486v1 2011-10-06,High-Precision Tuning of State for Memristive Devices by Adaptable Variation-Tolerant Algorithm,"Using memristive properties common for the titanium dioxide thin film devices, we designed a simple write algorithm to tune device conductance at a specific bias point to 1% relative accuracy (which is roughly equivalent to 7-bit precision) within its dynamic range even in the presence of large variations in switching behavior. The high precision state is nonvolatile and the results are likely to be sustained for nanoscale memristive devices because of the inherent filamentary nature of the resistive switching. The proposed functionality of memristive devices is especially attractive for analog computing with low precision data. As one representative example we demonstrate hybrid circuitry consisting of CMOS summing amplifier and two memristive devices to perform analog multiply and accumulate computation, which is a typical bottleneck operation in information processing.",1110.1393v1 2011-10-19,Evaluating the robustness of top coatings comprising plasma-deposited fluorocarbons in electrowetting systems,"Thin dielectric stacks comprising a main insulating layer and a hydrophobic top coating are commonly used in low voltage electrowetting systems. However, in most cases, thin dielectrics fail to endure persistent electrowetting testing at high voltages, namely beyond the saturation onset, as electrolysis indicates dielectric failure. Careful sample inspection via optical microscopy revealed possible local delamination of the top coating under high electric fields. Thus, improvement of the adhesion strength of the hydrophobic top coating to the main dielectric is attempted through a plasma-deposited fluorocarbon interlayer. Interestingly enough the proposed dielectric stack exhibited a) resistance to dielectric breakdown, b) higher contact angle modulation range, and c) electrowetting cycle reversibility. Appearance of electrolysis in the saturation regime is inhibited, suggesting the use of this hydrophobic dielectric stack for the design of more efficient electrowetting systems. The possible causes of the improved performance are investigated by nanoscratch characterization.",1110.4238v1 2011-10-21,P-T phase diagram of iron arsenide superconductor NdFeAsO0.88F0.12,"NdFeAsO0.88F0.12 belongs to the recently discovered family of high-TC iron-based superconductors. The influence of high pressure on transport properties of this material has been studied. Contrary to La-based compounds, we did not observe a maximum in TC under pressure. Under compression, TC drops rapidly as a linear function of pressure with the slope k = -2.8 \pm 0.1 K / GPa. The extrapolated value of TC at zero pressure is about TC (0) = 51.7 \pm 0.4 K. At pressures higher than ~18.4 GPa, the superconducting state disappears at all measured temperatures. The resistance changes slope and shows a turn-up behavior, which may be related to the Kondo effect or a weak localization of two-dimensional carriers below ~45 K that is above TC and thus competing with the superconducting phase. The behavior of the sample is completely reversible at the decompression. On the bases of our experimental data, we propose a tentative P-T phase diagram of NdFeAsO0.88F0.12.",1110.4909v1 2011-11-20,Flame Synthesis of Graphene Films in Open Environments,"Few-layer graphene (FLG) is grown on copper and nickel substrates at high rates using a novel flame synthesis method in open-atmosphere environments. Transmittance and resistance properties of the transferred films are similar to those grown by other methods, but the concentration of oxygen, as assessed by XPS, is actually less than that for CVD-grown graphene under near vacuum conditions. The method involves utilizing a multi-element inverse-diffusion-flame burner, where post-flame species and temperatures are radially-uniform upon deposition at a substrate. Advantages of the flame synthesis method are scalability for large-area surface coverage, increased growth rates, high purity and yield, continuous processing, and reduced costs due to efficient use of fuel as both heat source and reagent. Additionally, by adjusting local growth conditions, other carbon nanostructures (i.e. nanotubes) are readily synthesized.",1111.4699v1 2012-07-25,Conductivity crossover in nano-crystalline diamond films: Realization of a disordered superlattice-like structure,"We present the electrical transport characteristics of a batch of nano-crystalline diamond films of varying nitrogen concentrations and explain the conduction mechanism by the disordered quasi-superlattice model applied to semiconductor heterostructures. Synthesized by the hot filament chemical vapour deposition technique, the degree of structural disorder in the films, confirmed from Raman spectroscopy, is found to be controllable, resulting in the transition of conduction mechanism from localized and activated to the metallic conduction regime. Hence through high field magneto-resistance measurements at low temperatures we firmly establish a conductivity crossover from hopping to 3D weak localization. The long electronic dephasing time and its weak temperature dependence suggest the possibility for diamond-based high-speed device applications.",1207.5916v1 2012-10-23,Impact of the various spin and orbital ordering processes on multiferroic properties of orthovanadate DyVO3,"The orthovanadate DyVO3 crystal, known to exhibit multiple structural, spin and orbital ordering transitions, is presently investigated on the basis of magnetization, heat capacity, resistivity, dielectric and polarization measurements. Our main result is experimental evidence for the existence of multiferroicity below a high TC of 108 K over a wide temperature range including different spin-orbital ordered states. The onset of ferroelectricity is found to coincide with the antiferromagnetic C-type spin ordering transition taking place at 108 K, which indicates that DyVO3 belongs to type II multiferroics exhibiting a coupling between magnetism and ferroelectricity. Some anomalies detected on the temperature dependence of electric polarization are discussed with respect to the nature of the spin-orbital ordered states of the V sublattice and the degree of spin alignment in the Dy sublattice. The orthovanadates RVO3 (R = rare earth or Y) form an important new category for searching for high-TC multiferroics.",1210.6373v3 2013-04-04,Atomic Calligraphy: The Direct Writing of Nanoscale Structures using MEMS,"We present a micro-electromechanical system (MEMS) based method for the resist free patterning of nano-structures. Using a focused ion beam (FIB) to customize larger MEMS machines, we fabricate apertures as small as 50 nm on plates that can be moved with nanometer precision over an area greater than 20x20 {\mu}m^2. Depositing thermally evaporated gold atoms though the apertures while moving the plate results in the deposition of nanoscale metal patterns. Adding a shutter only microns above the aperture, enables high speed control of not only where but also when atoms are deposited. Using a shutter, different sized apertures can be selectively opened and closed for nano-structure fabrication with features ranging from nano- to micrometers in scale. The ability to evaporate materials with high precision, and thereby fabricate circuits and structures in situ, enables new kinds of experiments based on the interactions of a small number of atoms and eventually even single atoms.",1304.1334v1 2013-04-04,Substrate-Independent Catalyst-Free Synthesis of High-Purity Bi2Se3 Nanostructures,"We describe a catalyst-free vapor-solid synthesis of bismuth selenide (Bi2Se3) nanostructures at ambient pressure with hydrogen as a carrier gas. The nanostructures were synthesized on glass, silicon and mica substrates and the method yields a variety of nanostructures: nanowires, nanoribbons, nanoplatelets and nanoflakes. The materials analysis shows high chemical purity in all cases, without sacrificing the crystalline structure of Bi2Se3. Low-temperature measurements of the nanostructures indicate contributions from the surface states with a tunable carrier density. Samples synthesized on flexible mica substrates show no significant change in resistance upon bending, indicating robustness of as-grown Bi2Se3 nanostructures and their suitability for device applications.",1304.1388v1 2013-07-14,Voltage-triggered Ultra-fast Metal-insulator Transition in Vanadium Dioxide Switches,"Electrically driven metal-insulator transition in vanadium dioxide (VO2) is of interest in emerging memory devices, neural computation, and high speed electronics. We report on the fabrication of out-of-plane VO2 metal-insulator-metal (MIM) structures and reproducible high-speed switching measurements in these two-terminal devices. We have observed a clear correlation between electrically-driven ON/OFF current ratio and thermally-induced resistance change during metal-insulator transition. It is also found that sharp metal-insulator transition could be triggered by external voltage pulses within 2 ns at room temperature and the achieved ON/OFF ratio is greater than two orders of magnitude with good endurance.",1307.3774v1 2013-07-17,Dielectric Coatings for IACT Mirrors,"Imaging Atmospheric Cherenkov Telescopes for very-high energy gamma-ray astronomy need mirror with high reflectance roughly in the wavelength between 300 and 550 nm. The current standard reflective layer of such mirrors is aluminum. Being permanently exposed to the environment they show a constant degradation over the years. New and improved dielectric coatings have been developed to enhance their resistance to environmental impact and to extend their possible lifetime. In addition, these customized coatings have an increased reflectance of over 95% and are designed to significantly lower the night-sky background contribution. The development of such coatings for mirrors with areas up to 2 m2 and low application temperatures to suite the composite materials used for the new mirror susbtrates of the Cherenkov Telescope Array (CTA) and the results of extensive durability tests are presented.",1307.4557v1 2013-08-14,Perspectives of Micro-Pattern Gaseous Detector Technologies for Future Physics Projects,"A centenary after the invention of the basic principle of gas amplification, gaseous detectors - are still the first choice whenever the large area coverage with low material budget is required. Advances in photo-lithography and micro-processing techniques in the chip industry during the past two decades triggered a major transition in the field of gas detectors from wire structures to Micro-Pattern Gas Detector (MPGD) concepts, revolutionizing cell-size limitations for many gas detector applications. The high radiation resistance and excellent spatial and time resolution make them an invaluable tool to confront future detector challenges at the frontiers of research. The design of the new micro-pattern devices appears suitable for industrial production. In 2008, the RD51 collaboration at CERN has been established to further advance technological developments of MPGDs and associated electronic-readout systems, for applications in basic and applied research. This review provides an overview of the state-of-the-art of the MPGD technologies and summarizes recent activities for the next generation of colliders within the framework of the RD51 collaboration.",1308.3047v2 2013-08-18,Pulsed Laser Deposition of High-Quality Thin Films of the Insulating Ferromagnet EuS,"High-quality thin films of the ferromagnetic-insulator europium(II) sulfide (EuS) were fabricated by pulsed laser deposition on Al2O3 (0001) and Si (100) substrates. A single orientation was obtained with the [100] planes parallel to the substrates, with atomic-scale smoothness indicates a near-ideal surface topography. The films exhibit uniform ferromagnetism below 15.9 K, with a substantial component of the magnetization perpendicular to the plane of the films. Optimization of the growth condition also yielded truly insulating films with immeasurably large resistance. This combination of magnetic and electric properties open the gate for novel devices that require a true ferromagnetic insulator.",1308.3820v2 2014-02-19,Monte Carlo Simulation of RPC-based PET with GEANT4,"The Resistive Plate Chambers (RPC) are low-cost charged-particle detectors with good timing resolution and potentially good spatial resolution. Using RPC as gamma detector provides an opportunity for application in positron emission tomography (PET). In this work, we use GEANT4 simulation package to study various methods improving the detection efficiency of a realistic RPC-based PET model for 511keV photons, by adding more detection units, changing the thickness of each layer, choosing different converters and using multi-gaps RPC (MRPC) technique. Proper balance among these factors are discussed. It's found that although RPC with materials of high atomic number can reach a higher efficiency, they may contribute to a poor spatial resolution and higher background level.",1402.4544v1 2014-03-04,Molecular weight dependent bimolecular recombination in organic solar cells,"Charge carrier recombination is studied in operational organic solar cells made from the polymer:fullerene system PCDTBT:PC71BM (poly[N-9""-heptadecanyl-2,7-carbazole-alt-5,5-(4',7'-di-2-thienyl-2',1',3'-benzothiadiazole)] : [6,6]-phenyl-C$_{70}$-butyric acid methyl ester). A newly developed technique High Intensity Resistance dependent PhotoVoltage (HI-RPV) is presented for reliably quantifying the bimolecular recombination coefficient independently of variations in experimental conditions, thereby resolving key limitations of previous experimental approaches. Experiments are performed on solar cells of varying thicknesses and varying polymeric molecular weights. It is shown that solar cells made from low molecular weight PCDTBT exhibit Langevin recombination, whereas suppressed (non-Langevin) recombination is found in solar cells made with high molecular weight PCDTBT.",1403.0972v2 2015-01-27,Transition from semiconducting to metallic-like conducting and weak antilocalization effect in single crystals of LuPtSb,"High quality half-Heusler single crystals of LuPtSb have been synthesized by a Pb flux method. The temperature dependent resistivity and Hall effects indicate that the LuPtSb crystal is a p-type gapless semiconductor showing a transition from semiconducting to metallic conducting at 150 K. Moreover, a weakly temperature-dependent positive magnetoresistance (MR) as large as 109 % and high carrier mobility up to 2950 cm2/Vs are experimentally observed at temperatures below 150 K. The low-field MR data shows evidence for weak antilocalization (WAL) effect at temperatures even up to 150 K. Analysis of the temperature and angle dependent magnetoconductance manifests that the WAL effect originates from the bulk contribution owing to the strong spin-orbital coupling.",1501.06714v1 2015-05-22,Synthesis of monoclinic IrTe2 under high pressure and its physical properties,"In a pressure-temperature (P-T) diagram for synthesizing IrTe2 compounds, the well-studied trigonal (H) phase with the CdI2-type structure is stable at low pressures. The superconducting cubic (C) phase can be synthesized under higher temperatures and pressures. A rhombohedral phase with the crystal structure similar to the C phase can be made at ambient pressure; but the phase contains a high concentration of Ir deficiency. In this paper, we report that a rarely studied monoclinic (M) phase can be stabilized in narrow ranges of pressure and temperature in this P-T diagram. The peculiar crystal structure of the M-IrTe2 eliminates the tendency to form Ir-Ir dimers found in the H phase. The M phase has been fully characterized by structural determination and measurements of electrical resistivity, thermoelectric power, DC magnetization, and specific heat. These physical properties have been compared with those in the H and C phases of Ir1-xTe2. Moreover, magnetic and transport properties and specific heat of the M-IrTe2 can be fully justified by calculations with the density-functional theory presented in this paper.",1505.06124v1 2015-08-12,Direct Observation of Re-entrant Multiferroic CuO at High Pressures,"We have carried out a detailed experimental investigation on CuO using dielectric constant, ac resistance, Raman spectroscopy and X-ray diffraction measurements at high pressures and room temperature. Both dielectric constant and dielectric loss show an anomalous peak in the pressure range 3.4-4 GPa indicating a ferroelectric transition. Raman studies show anomalous behaviour of the Ag mode with a slope change in the mode frequency and a minimum in the mode FWHM at 3.4 GPa indicating a strong spin phonon coupling along [1 0 -1] direction. A step like behaviour in the intensity of the Ag mode is observed at 3.4 GPa, indicating a change in the polarization of the mode. A maximum in the intensity of (2,0,-2)Bragg peak at 3.4 GPa points the occurrence of critical scattering due to emergence of magnetic exchange interaction. All our experimental evidences show to the presence of re-entrant type-II multiferroic behaviour in CuO at about 4 GPa.",1508.02874v1 2015-10-21,Titanium Nitride as a Seed Layer for Heusler Compounds,"Titanium nitride (TiN) shows low resistivity at room temperature, high thermal stability and thus has the potential to serve as seed layer in magnetic tunnel junctions. High quality TiN thin films with regard to the crystallographic and electrical properties were grown and characterized by X-ray diffraction and 4-terminal transport measurements. Element specific X-ray absorption spectroscopy revealed pure TiN in the bulk. To investigate the influence of a TiN seed layer on a ferro(i)magnetic bottom electrode, an out-of-plane magnetized Mn2.45Ga as well as in- and out-of-plane magnetized Co2FeAl thin films were deposited on a TiN buffer, respectively. The magnetic properties were investigated using a superconducting quantum interference device (SQUID) and anomalous Hall effect (AHE) for Mn2.45Ga. Magneto optical Kerr effect (MOKE) measurements were carried out to investigate the magnetic properties of Co2FeAl. TiN buffered Mn2.45Ga thin films showed higher coercivity and squareness ratio compared to unbuffered samples. The Heusler compound Co2FeAl showed already good crystallinity when grown at room temperature.",1510.06256v3 2016-04-19,Insulating and metallic spin glass in K$_{x}$Fe$_{2-δ-y}$Ni$_{y}$Se$_{2}$ (0.06 $\leq$ $y$ $\leq$ 1.44) single crystals,"We report electron doping effects by Ni in K$_{x}$Fe$_{2-\delta-y}$Ni$_{y}$Se$_{2}$ (0.06 $\leq$ $y$ $\leq$ 1.44) single crystal alloys. A rich ground state phase diagram is observed. Small amount of Ni ($\sim$ 4\%) suppressed superconductivity below 1.8 K, inducing insulating spin glass magnetic ground state for higher Ni content. With further Ni substitution, metallic resistivity is restored. For high Ni concentration in the lattice the unit cell symmetry is high symmetry $I4/mmm$ with no phase separation whereas both $I4/m + I4/mmm$ space groups were detected in the phase separated crystals when concentration of Ni $<$ Fe. The absence of superconductivity coincides with the absence of crystalline Fe vacancy order.",1604.05713v1 2016-05-16,Growth and characterization of CaFe$_{1-x}$Co$_x$AsF single crystals by CaAs flux method,"Millimeter sized single crystals of CaFe$_{1-x}$Co$_x$AsF were grown using a self-flux method. It is found that high-quality single crystals can be grown from three approaches with different initial raw materials. The chemical compositions and crystal structure were characterized carefully. The c-axis lattice constant is suppressed by the Co substitution. Superconductivity with the critical transition $T_c$ as high as 21 K was confirmed by both the resistivity and magnetic susceptibility measurements in the sample with $x$ = 0.12. Moreover, it is found that $T_c$ can be enhanced for about 1 K under the very small hydrostatic pressure of 0.22 GPa, which is more quickly than that reported in the polycrystalline samples. Our results is a promotion for the physical investigations of 1111 phase iron-pnictide superconductors.",1605.04642v1 2016-06-02,High Current Density 2D/3D Esaki Tunnel Diodes,"The integration of two-dimensional materials such as transition metal dichalcogenides with bulk semiconductors offer interesting opportunities for 2D/3D heterojunction-based novel device structures without any constraints of lattice matching. By exploiting the favorable band alignment at the GaN/MoS2 heterojunction, an Esaki interband tunnel diode is demonstrated by transferring large area, Nb-doped, p-type MoS2 onto heavily n-doped GaN. A peak current density of 446 A/cm2 with repeatable room temperature negative differential resistance, peak to valley current ratio of 1.2, and minimal hysteresis was measured in the MoS2/GaN non-epitaxial tunnel diode. A high current density of 1 kA/cm2 was measured in the Zener mode (reverse bias) at -1 V bias. The GaN/MoS2 tunnel junction was also modeled by treating MoS2 as a bulk semiconductor, and the electrostatics at the 2D/3D interface was found to be crucial in explaining the experimentally observed device characteristics.",1606.00509v1 2016-06-24,Thermal insulator transition induced by interface scattering,"We develop an effective medium model of thermal conductivity that accounts for both percolation and interface scattering. This model accurately explains the measured increase and decrease of thermal conductivity with loading in composites dominated by percolation and interface scattering, respectively. Our model further predicts that strong interface scattering leads to a sharp decrease in thermal conductivity, or an insulator transition, at high loadings when conduction through the matrix is restricted and heat is forced to diffuse through particles with large interface resistance. The accuracy of our model and its ability to predict transitions between insulating and conducting states suggest it can be a useful tool for designing materials with low or high thermal conductivity for a variety of applications.",1606.07851v2 2016-06-29,Large linear magnetoresistance from neutral defects in Bi$_2$Se$_3$,"The chalcogenide Bi$_2$Se$_3$ can attain the three dimensional (3D) Dirac semimetal state under the influence of strain and microstrain. Here we report the presnece of large linear magnetoresistance in such a Bi$_2$Se$_3$ crystal. The magnetoresistance has quadratic form at low fields which crossovers to linear above 4 T. The temperature dependence of magnetoresistance scales with carrier mobility and the crossover field scales with inverse of mobility. Our analysis suggest that the linear magnetoresistance in our system has a classical origin and arises from the scattering of high mobility 3D Dirac electrons from crystalline inhomogeneities. We observe that the charged selenium vacancies are strongly screened by high mobility Dirac electrons and the neutral crystalline defects are the main scattering center for transport mechanism. Our analysis suggests that both the resistivity and the magnetoresistance have their origin in scattering of charge carriers from neutral defects.",1606.09059v1 2016-10-03,Thallium under extreme compression,"We present a combined theoretical and experimental study of the high-pressure behavior of thallium. X-ray diffraction experiments have been carried out at room temperature up to 125 GPa using diamond-anvil cells, nearly doubling the pressure range of previous experiments. We have confirmed the hcp-fcc transition at 3.5 GPa and determined that the fcc structure remains stable up to the highest pressure attained in the experiments. In addition, HP-HT experiments have been performed up to 8 GPa and 700 K by using a combination of x-ray diffraction and a resistively heated diamond-anvil cell. Information on the phase boundaries is obtained, as well as crystallographic information on the HT bcc phase. The equation of state for different phases is reported. Ab initio calculations have also been carried out considering several potential high-pressure structures. They are consistent with the experimental results and predict that, among the structures considered in the calculations, the fcc structure of thallium is stable up to 4.3 TPa. Calculations also predict the post-fcc phase to have a close-packed orthorhombic structure above 4.3 TPa.",1610.00435v1 2016-10-19,Applications and non-idealities of submicron Al-AlOx-Nb tunnel junctions,"We have developed a technique to fabricate sub-micron, 0.6 um x 0.6 um Al-AlOx-Nb tunnel junctions using a standard e-beam resist, angle evaporation and double oxidation of the tunneling barrier, resulting in high quality niobium, as determined by the the high measured values of the critical temperature TC 7.5 K and the gap 1.3 meV. The devices show great promise for local nanoscale thermometry in the temperature range 1 - 7.5 K. Electrical characterization of the junctions was performed at sub-Kelvin temperatures both with and without an external magnetic field, which was used to suppress superconductivity in Al and thus bring the junction into a normal-metal-insulator-superconductor (NIS) configuration. We observed excess sub-gap current, which could not be explained by the standard tunneling theory. Evidence points towards materials science issues of the barrier or Nb/AlOx interface as the culprit.",1610.05903v1 2017-06-28,Super-Hydrophobic Stearic Acid Layer Formed on Anodized High Purified Magnesium for Improving Corrosion Resistance of Biodegradable Implants,"Magnesium and its alloys are ideal candidates for biodegradable implants. However, they can dissolve too rapidly in the human body for most applications. In this research, high purified magnesium (HP-Mg) was coated with stearic acid in order to slow the corrosion rate of magnesium in simulated body fluid at 37{\deg}C. HP-Mg was anodized to form an oxide/hydroxide layer, then it was immersed in a stearic acid solution. Electrochemical impedance spectroscopy and potentiodynamic polarization were used to estimate the corrosion rate of HP-Mg specimens. The results confirm that the hydrophobic coating can temporarily decrease the corrosion rate of HP-Mg by 1000x.",1706.09508v1 2017-10-19,Design of high-strength refractory complex solid-solution alloys,"Nickel-based superalloys and near-equiatomic high-entropy alloys containing Molybdenum are known for higher temperature strength and corrosion resistance. Yet, complex solid-solution alloys offer a huge design space to tune for optimal properties at slightly reduced entropy. For refractory Mo-W-Ta-Ti-Zr, we showcase KKR electronic-structure methods via the coherent-potential approximation to identify alloys over 5-dimensional design space with improved mechanical properties and necessary global (formation enthalpy) and local (short-range order) stability. Deformation is modeled with classical molecular dynamic simulations, validated from our first-principles data. We predict complex solid-solution alloys of improved stability with greatly enhanced modulus of elasticity ($3\times$ at 300 K) over near-equiatomic cases, as validated experimentally, and with higher moduli above 500~K over commercial alloys ($2.3\times$ at 2000 K). We also show that optimal complex solid-solution alloys are not described well by classical potentials due to critical electronic effects.",1710.06983v2 2017-11-16,Superconductivity at 7.3 K in the 133-type Cr-based RbCr3As3 single crystals,"Here we report the preparation and superconductivity of the 133-type Cr-based quasi-one-dimensional (Q1D) RbCr3As3 single crystals. The samples were prepared by the deintercalation of Rb+ ions from the 233-type Rb2Cr3As3 crystals which were grown from a high-temperature solution growth method. The RbCr3As3 compound crystallizes in a centrosymmetric structure with the space group of P63/m (No. 176) different with its non-centrosymmetric Rb2Cr3As3 superconducting precursor, and the refined lattice parameters are a = 9.373(3) {\AA} and c = 4.203(7) {\AA}. Electrical resistivity and magnetic susceptibility characterizations reveal the occurrence of superconductivity with an interestingly higher onset Tc of 7.3 K than other Cr-based superconductors, and a high upper critical field Hc2(0) near 70 T in this 133-type RbCr3As3 crystals.",1711.06133v1 2017-12-01,Radiation damage and thermal shock response of carbon-fiber-reinforced materials to intense high-energy proton beams,"A comprehensive study on the effects of energetic protons on carbon-fiber composites and compounds under consideration for use as low-Z pion production targets in future high-power accelerators and low-impedance collimating elements for intercepting TeV-level protons at the Large Hadron Collider has been undertaken addressing two key areas, namely, thermal shock absorption and resistance to irradiation damage.",1712.00509v1 2018-01-08,Automated Instrumentation for the Determination of the High-Temperature Thermoelectric Figure-of-Merit,"In this work, we report the fabrication of a high temperature measurement setup to measure Figure of merit (ZT). This setup facilitates the simultaneous measurement of Seebeck coefficient ({\alpha}), thermal conductivity (\kappa), and electrical resistivity (\rho) required to calculate ZT. Measurement of temperature, as well as voltages using same thermocouples, simplified the design of the setup by minimizing sensors and wires. Limited components used in the sample holder further simplify the design and make it small in size and lightweight. The dedicated thin heater is made, which minimizes the heat loss. Further, low heat loss is achieved by optimizing the insulator dimension. To measure power delivered to the heater, 4-wire technique is used. Low cost and commonly available materials used in the fabrication of various components make it more accessible to the user as any parts can be easily replaced in case of any damage occurs. A dedicated program is built in the Python programming language to automate the whole measurement process. p-type Bi0.36Sb1.45Te3 sample is used to calibrate this measurement setup. The data collected are found to be in good agreement with the reported data.",1801.02360v1 2018-01-30,Structural and electronic phase transitions in FePS$_3$ under the application of pressure,"Two-dimensional materials have proven to be a prolific breeding ground of new and unstudied forms of magnetism and unusual metallic states, particularly when tuned between their insulating and metallic phases. In this paper we present work on a new metal to insulator transition system FePS$_3$ . This compound is a two-dimensional van-der-Waals antiferromagnetic Mott insulator. Here we report the discovery of an insulator-metal transition in FePS$_3$, as evidenced by x-ray diffraction and electrical transport measurements, using high pressure as a tuning parameter. Two structural phase transitions are observed in the x-ray diffraction data as a function of pressure and resistivity measurements show evidence of onset of a metallic state at high pressures. We propose models for the two new structures that can successfully explain the x-ray diffraction patterns.",1801.10089v2 2018-03-14,A 1.6:1 Bandwidth Two-Layer Antireflection Structure for Silicon Matched to the 190-310 GHz Atmospheric Window,"Although high-resistivity, low-loss silicon is an excellent material for THz transmission optics, its high refractive index necessitates antireflection treatment. We fabricated a wide-bandwidth, two-layer antireflection treatment by cutting subwavelength structures into the silicon surface using multi-depth deep reactive ion etching (DRIE). A wafer with this treatment on both sides has <-20 dB (<1%) reflectance over 190-310 GHz. We also demonstrated that bonding wafers introduces no reflection features above the -20 dB level, reproducing previous work. Together these developments immediately enable construction of wide-bandwidth silicon vacuum windows and represent two important steps toward gradient-index silicon optics with integral broadband antireflection treatment.",1803.05168v2 2018-04-26,Large effective mass and interaction-enhanced Zeeman splitting of $K$-valley electrons in MoSe$_2$,"We study the magnetotransport of high-mobility electrons in monolayer and bilayer MoSe$_2$, which show Shubnikov-de Haas (SdH) oscillations and quantum Hall states in high magnetic fields. An electron effective mass of 0.8$m_e$ is extracted from the SdH oscillations' temperature dependence; $m_e$ is the bare electron mass. At a fixed electron density the longitudinal resistance shows minima at filling factors (FFs) that are either predominantly odd, or predominantly even, with a parity that changes as the density is tuned. The SdH oscillations are insensitive to an in-plane magnetic field, consistent with an out-of-plane spin orientation of electrons at the $K$-point. We attribute the FFs parity transitions to an interaction enhancement of the Zeeman energy as the density is reduced, resulting in an increased Zeeman-to-cyclotron energy ratio.",1804.10104v2 2018-05-31,Unusual magnetotransport in holmium monoantimonide,"We report the magnetotransport properties of HoSb, a semimetal with antiferromagnetic ground state. HoSb shows extremely large magnetoresistance (XMR) and Shubnikov-de Haas (SdH) oscillation at low temperature and high magnetic field. Different from previous reports in other rare earth monopnictides, kinks in $\rho(B)$ and $\rho_{xy}(B)$ curves and the field dependent resistivity plateau are observed in HoSb, which result from the magnetic phase transitions. The fast Fourier transform analysis of the SdH oscillation reveals the split of Fermi surfaces induced by the nonsymmetric spin-orbit interaction. The Berry phase extracted from SdH oscillation indicates the possible nontrivial electronic structure of HoSb in the presence of magnetic field. The Hall measurements suggest that the XMR originates from the electron-hole compensation and high mobility.",1805.12496v1 2018-06-28,Tribological Properties of Ultrananocrystalline Diamond Nanowire Thin Film: Influence of Sliding Ball Counterbodies,"Ultrananocrystalline Diamond Nanowire (UNCD NW) thin film was deposited on mirror polished silicon substrate (100) using Microwave Plasma Enhanced Chemical Vapor Deposition (MPECVD) System with optimized deposition parameters in CH4 (6%)/N2 plasma media. The film exhibited wire like morphology with randomly oriented and homogeneously distributed ultranano diamond grains separated by an interphase boundary of graphitic and amorphous carbon (a-C) phases. Micro-tribological studies of film were carried out against Al2O3, SiC and steel balls in ambient atmospheric conditions. Initially, the friction coefficient was found to be high for UNCD NW/SiC and UNCD NW/Steel sliding pairs which gradually decreased to low value. While, in UNCD NW/Al2O3 sliding combination, the ultralow value of friction coefficient was maintained throughout the whole sliding process. High wear resistant properties of the film were observed in UNCD NW/SiC and UNCD NW/Steel pairs. In UNCD NW/Al2O3 case, ball counterbody showed negligible wear dimension. Such kind of tribological behavior was attributed to the different type of mechanical and chemical interactions of ball counterbodies with UNCD NW thin film.",1806.10765v1 2018-09-13,Anisotropic hybridization in a new Kondo lattice compound CeCoInGa$_3$,"We report a detailed and comparative study of the single crystal CeCoInGa$_3$ in both experiment and theory. Resistivity measurements reveal the typical behavior of Kondo lattice with the onset temperature of coherence, $T^*\approx 50\,$K. The magnetic specific heat can be well fitted using a spin-fluctuation model at low temperatures, yielding a large Sommerfeld coefficient, $\gamma\approx172\,$mJ/mol K$^2$ at 6 K, suggesting that this is a heavy-fermion compound with a pronounced coherence effect. The magnetic susceptibility exhibits a broad field-independent peak at $T_{\chi}$ and shows an obvious anisotropy within the $bc$ plane, reflecting the anisotropy of the coherence effect at high temperatures. These are compared with strongly correlated calculations combining first-principles band structure calculations and dynamical mean-field theory. Our results confirm the onset of coherence at about 50 K and reveal a similar anisotropy in the hybridization gap, pointing to a close connection between the hybridization strength of the low-temperature Fermi-liquid state and the high-temperature coherence effect.",1809.04735v1 2018-11-18,In situ high-cycle fatigue reveals the importance of grain boundary structure in nanocrystalline Cu-Zr,"Nanocrystalline metals typically have high fatigue strengths, but low resistance to crack propagation. Amorphous intergranular films are disordered grain boundary complexions that have been shown to delay crack nucleation and slow crack propagation during monotonic loading by diffusing grain boundary strain concentrations, suggesting they may also be beneficial for fatigue properties. To probe this hypothesis, in situ transmission electron microscopy fatigue cycling is performed on Cu-1 at.% Zr thin films thermally treated to have either only ordered grain boundaries or to contain amorphous intergranular films. The sample with only ordered grain boundaries experienced grain coarsening at crack initiation followed by unsteady crack propagation and extensive nanocracking, whereas the sample containing amorphous intergranular films had no grain coarsening at crack initiation followed by steady crack propagation and distributed plastic activity. Microstructural design for control of these behaviors through simple thermal treatments can allow for the improvement of nanocrystalline metal fatigue toughness.",1811.07263v1 2019-09-02,Thermoelastic equation of state and melting of Mg metal at high pressure and high temperature,"The p-V-T equation of state of magnesium metal has been measured up to 20 GPa and 1500 K using both multianvil and opposite anvil techniques combined with synchrotron X-ray diffraction. To fit the experimental data, the model of Anderson-Gr\""uneisen has been used with fixed parameter {\delta}T. The 300-K bulk modulus of B0 = 32.5(1) GPa and its first pressure derivative, B0' = 3.73(2), have been obtained by fitting available data up to 20 GPa to Murnaghan equation of state. Thermal expansion at ambient pressure has been described using second order polynomial with coefficients a = 25(2)x10-6 K-1 and b = 9.4(4)x10-9 K-2. The parameter describing simultaneous pressure and temperature impact on thermal expansion coefficient (and, therefore, volume) is {\delta}T = 1.5(5). The good agreement between fitted and experimental isobars has been achieved to relative volumes of 0.75. The Mg melting observed by X-ray diffraction and in situ electrical resistivity measurements confirms previous results and additionally confirms the p-T estimations in the vicinity of melting.",1909.00645v1 2014-08-28,Crossover of conduction mechanism in Sr2IrO4 epitaxial thin films,"High quality epitaxial Sr2IrO4 thin films with various thicknesses (9-300 nm) have been grown on SrTiO3 (001) substrates, and their electric transport properties have been investigated. All samples showed the expected insulating behavior with a strong resistivity dependence on film thickness, that can be as large as three orders of magnitude at low temperature. A close examination of the transport data revealed interesting crossover behaviors for the conduction mechanism upon variation of thickness and temperature. While Mott variable range hopping (VRH) dominated the transport for films thinner than 85 nm, high temperature thermal activation behavior was observed for films with large thickness, which was followed by a crossover from Mott to Efros-Shklovskii (ES) VRH in the low temperature range. This low temperature crossover from Mott to ES VRH indicates the presence of a Coulomb gap (~3 meV). Our results demonstrate the competing and tunable conduction in Sr2IrO4 thin films, which in turn would be helpful for understanding the insulating nature related to strong spin-orbit-coupling of the 5d iridates.",1408.6798v1 2017-03-01,Tunnel-injected sub-260 nm ultraviolet light emitting diodes,"We report on tunnel-injected deep ultraviolet light emitting diodes (UV LEDs) configured with a polarization engineered Al0.75Ga0.25N/ In0.2Ga0.8N tunnel junction structure. Tunnel-injected UV LED structure enables n-type contacts for both bottom and top contact layers. However, achieving Ohmic contact to wide bandgap n-AlGaN layers is challenging and typically requires high temperature contact metal annealing. In this work, we adopted a compositionally graded top contact layer for non-alloyed metal contact, and obtained a low contact resistance of Rc=4.8x10-5 Ohm cm2 on n-Al0.75Ga0.25N. We also observed a significant reduction in the forward operation voltage from 30.9 V to 19.2 V at 1 kA/cm2 by increasing the Mg doping concentration from 6.2x1018 cm-3 to 1.5x1019 cm-3. Non-equilibrium hole injection into wide bandgap Al0.75Ga0.25N with Eg>5.2 eV was confirmed by light emission at 257 nm. This work demonstrates the feasibility of tunneling hole injection into deep UV LEDs, and provides a novel structural design towards high power deep-UV emitters.",1703.00117v1 2019-02-27,High-performance dendritic metamaterial absorber for broadband and near-meter wave radar,"Absorbing materials in ultra-high frequency (UHF) band has constantly been a major challenge. The size of the absorber in UHF band is large, whereas the resonant frequency band is narrow. According to Rozanov's theory, two kinds of composite metamaterial absorbers are designed to realize the requirements of low-frequency broadband metamaterial microwave absorber: the magnetic-metamaterial composite absorber1 (MA1) and the dielectric-metamaterial composite absorber 2 (MA2). In the range of approximately 300-1000MHz, both absorbers achieve absorption of over 90% and feature good adaptability to the incident angle of the incident wave. The absorbers also present good absorption rate of over 80% in the range of 0-45 degree. Processing samples of indium tin oxide (ITO) resistance film and polymethacrylimide (PMI) foam board feature simple preparation and low cost, and the most important thing is to consider the weight problem, which features certain advantages in terms of use.",1902.10398v1 2019-07-29,Mechanical Characterisation of the Protective Al$_2$O$_3$ Scale in Cr$_2$AlC MAX phases,"MAX phases have great potential under demands of both high-temperature and high-stress performance, with their mixed atomic bonding producing the temperature and oxidation resistance of ceramics with the mechanical resilience of metals. Here, we measure the mechanical properties up to 980C by nanoindentation on highly dense and pure Cr$_2$AlC, as well as after oxidation with a burner rig at 1200C for more than 29 hours. Only modest reductions in both hardness and modulus up to 980C were observed, implying no change in deformation mechanism. Furthermore, micro-cantilever fracture tests were carried out at the Cr$_2$AlC/Cr$_7$C$_3$ and Cr$_7$C$_3$/Al$_2$O$_3$ interfaces after the oxidation of the Cr$_2$AlC substrates with said burner rig. The values are typical of ceramic-ceramic interfaces, below 4 MPa/m, leading to the hypothesis that the excellent macroscopic behaviour is due to a combination of low internal strain due to the match in thermal expansion coefficient as well as the convoluted interface.",1907.12341v1 2019-03-21,Stabilization and heteroepitaxial growth of metastable tetragonal FeS thin films by pulsed laser deposition,"Pulsed laser deposition, a non-equilibrium thin-film growth technique, was used to stabilize metastable tetragonal iron sulfide (FeS), the bulk state of which is known as a superconductor with a critical temperature of 4 K. Comprehensive experiments revealed four important factors to stabilize tetragonal FeS epitaxial thin films: (i) an optimum growth temperature of 300 {\deg}C followed by thermal quenching, (ii) an optimum growth rate of ~7 nm/min, (iii) use of a high-purity bulk target, and (iv) use of a single-crystal substrate with small in-plane lattice mismatch (CaF2). Electrical resistivity measurements indicated that none of all the films exhibited superconductivity. Although an electric double-layer transistor structure was fabricated using the tetragonal FeS epitaxial film as a channel layer to achieve high-density carrier doping, no phase transition was observed. Possible reasons for the lack of superconductivity include lattice strain, off-stoichiometry of the film, electrochemical etching by the ionic liquid under gate bias, and surface degradation during device fabrication.",1903.08820v1 2019-03-26,Gate tunable quantum Hall effects in defect-suppressed Bi2Se3 films,"Despite many years of efforts, attempts to reach the quantum regime of topological surface states (TSS) on an electrically tunable topological insulator (TI) platform have so far failed on binary TI compounds such as Bi2Se3 due to high density of interfacial defects. Here, utilizing an optimal buffer layer on a gatable substrate, we demonstrate the first electrically tunable quantum Hall effects (QHE) on TSS of Bi2Se3. On the n-side, well-defined QHE shows up, but it diminishes near the charge neutrality point (CNP) and completely disappears on the p-side. Furthermore, around the CNP the system transitions from a metallic to a highly resistive state as the magnetic field is increased, whose temperature dependence indicates presence of an insulating ground state at high magnetic fields.",1903.10945v2 2019-04-09,Alloy Design for Mechanical Properties: Conquering the Length Scales,"Predicting the structural response of advanced multiphase alloys and understanding the underlying microscopic mechanisms that are responsible for it are two critically important roles modeling plays in alloy development. An alloys demonstration of superior properties, such as high strength, creep resistance, high ductility, and fracture toughness, is not sufficient to secure its use in widespread application. Still, a good model is needed, to take measurable alloy properties, such as microstructure and chemical composition, and forecast how the alloy will perform in specified mechanical deformation conditions, including temperature, time, and rate. In this bulletin, we highlight recent achievements by multiscale modeling in elucidating the coupled effects of alloying, microstructure, and the dynamics of mechanisms on the mechanical properties of polycrystalline alloys. Much of the understanding gained by these efforts relied on integration of computational tools that varied over many length and time scales, from first principles density functional theory, atomistic simulation methods, dislocation and defect theory, micromechanics, phase field modeling, single crystal plasticity, and polycrystalline plasticity.",1904.04569v1 2019-08-13,Investigating the real-time dissolution of a compositionally complex alloy using inline ICP and correlation with XPS,"The real-time dissolution of the single-phase compositionally complex alloy (CCA), Al1.5TiVCr, was studied using an inline inductively coupled plasma method. Compositionally complex alloys (CCAs), a term encompassing high entropy alloys (HEAs) or multi-principal element alloys (MPEAs), are - in general - noted for their inherently high corrosion resistance. In order to gain an insight into the dissolution of Al1.5TiVCr alloy, atomic emission spectroelectrochemistry was utilised in order to measure the ion dissolution of the alloy during anodic polarisation. It was revealed that incongruent dissolution occurred, with preferential dissolution of Al, and essentially no dissolution of Ti, until the point of alloy breakdown. Results were correlated with X-ray photoelectron spectroscopy, which revealed a complex surface oxide inclusive of unoxidised metal, and metal oxides in disproportion to the bulk alloying element ratio.",1908.04493v1 2012-06-01,Quantum Superinductor with Tunable Non-Linearity,"We report on the realization of a superinductor, a dissipationless element whose microwave impedance greatly exceeds the resistance quantum. The design of the superinductor, implemented as a ladder of nanoscale Josephson junctions, enables tuning of the inductance and its nonlinearity by a weak magnetic field. The Rabi decay time of the superinductor-based qubit exceeds 1 microsecond. The high kinetic inductance and strong nonlinearity offer new types of functionality, including the development of qubits protected from both flux and charge noises, fault tolerant quantum computing, and high-impedance isolation for electrical current standards based on Bloch oscillations.",1206.0307v2 2015-07-10,Antibunched photons from inelastic Cooper-pair tunneling,"We demonstrate theoretically that charge transport across a Josephson junction, voltage-biased through a resistive environment, produces antibunched photons. We develop a continuous-mode description of the emitted radiation field in a semi-infinite transmission line terminated by the Josephson junction. Within a perturbative treatment in powers of the tunneling coupling across the Josephson junction, we capture effects originating in charging dynamics of consecutively tunneling Cooper pairs. We find that within a feasible experimental setup the Coulomb blockade provided by high zero-frequency impedance can be used to create antibunched photons at a very high rate and in a very versatile frequency window ranging from a few GHz to a THz.",1507.02885v1 2018-07-20,High-Pressure Phase Diagram of NdFeAsO$_{0.9}$F$_{0.1}$: Disappearance of superconductivity on the verge of ferromagnetism from nd moments,"We investigated transport and magnetic properties of NdFeAsO$_{0.9}$F$_{0.1}$ single crystal under hydrostatic pressures up to 50\,GPa. The ambient pressure superconductivity at $T_{c} \sim$ 45.4\,K is fully suppressed at $P_{c} \sim$ 21 GPa. Upon further increase of the pressure, the ferromagnetism associated with the order of rare-earth subsystem is induced at the border of superconductivity. Our finding is supported by the hysteresis in the magnetization $M$($H$) loops and the strong increase in the field cooled data, $M$($T$), toward low temperatures. We also show that the temperature evolution of the electrical resistivity as a function of pressure is consistent with a crossover from a Fermi-liquid to non-Fermi-liquid to Fermi-liquid. These results give access to the high-pressure side of the superconducting phase diagram in 1111 type of materials.",1807.07729v1 2018-12-19,Benchmarking vdW-DF first principle predictions against Coupled Electron-Ion Monte Carlo for high pressure liquid hydrogen,"We report first principle results for nuclear structure and optical responses of high pressure liquid hydrogen along two isotherms in the region of molecular dissociation. We employ Density Functional Theory with the vdW-DF approximation (vdW) and we benchmark the results against existing predictions from Coupling Electron-Ion Monte Carlo (CEIMC). At fixed density and temperature, we find that pressure from vdW is higher than pressure from CEIMC by about 10 GPa in the molecular insulating phase and about 20 GPa in the dissociated metallic phase. Molecules are found to be overstabilized using vdW, with a slightly shorter bond length, and with a stronger resistance to compression. As a consequence, pressure dissociation along isotherms using vdW is more progressive than computed with CEIMC. Below the critical point, the liquid-liquid phase transition is observed with both theories in the same density region but the one predicted by vdW has a smaller density discontinuity, i.e. a smaller first order character. The optical conductivity computed using Kubo-Greenwood is rather similar for the two systems and reflects the slightly more pronounced molecular character of vdW.",1812.07818v1 2019-10-01,In-situ detection of nucleation in high temperature solutions,"The state of a sample during crystal growth from high temperature solutions is not accessible in conventional furnace systems. An optimization of the growth parameters often requires arduous trial and error procedures in particular in case of novel multicomponent systems with unknown phase diagrams. Here we present a measurement technique based on lock-in amplification that allows for in-situ detection of the liquidus and solidus temperatures as well as structural phase transitions. A thin, metallic measurement wire is mounted in close vicinity to the melt. Characteristic anomalies in the time-dependent electrical resistivity of this wire allow for the detection of latent heat release without using a reference crucible. The method is implemented in a 'feedback furnace' and enables an adjustment of the temperature profile based on the occurrence or absence of phase transitions. The absolute temperature serves as an additional source of information. Obtained phase transition temperatures are in good agreement with differential thermal analysis (DTA).",1910.00316v1 2019-10-04,Improvement of temperature uniformity of induction-heated T-shape susceptor for high-temperature MOVPE,"The induction heating is a common method applied in metalorganic vapor phase epitaxy (MOVPE) especially for higher-temperature growth conditions. However, compared to the susceptor heated by the multiple-zone resistant heater, the inductive-heated susceptor could suffer from severe thermal non-uniformity issue. In this simulation study, we propose to employ a T-shape susceptor design with various geometric modifications to significantly improve the substrate temperature uniformity by manipulating thermal transfer. Specifically, the thermal profile can be tailored by horizontal expansion and vertical elongation of the susceptor, or forming a cylindrical hollow structure at the susceptor bottom cylinder. Three optimized designs are shown with different temperature uniformity as well as various induction heating efficiencies. The temperature variation of the entire substrate surface can be less than 5 {\deg}C at ~1900 {\deg}C with high induction heating efficiency after applying the proposed techniques.",1910.02024v1 2019-10-21,Harnessing energy landscape exploration to control the buckling of cylindrical shells,"The complexity and unpredictability of postbuckling responses in even simple thin shells have raised great challenges to emerging technologies exploiting buckling transitions. Here we comprehensively survey the buckling landscapes to show the full complexity of the stable buckling states and the transition mechanisms between each of them. This is achieved by combining a simple and versatile triangulated lattice model for modelling the shell morphologies with efficient high-dimensional free-energy minimisation and transition path finding algorithms. We show how the simple free energy landscapes of short, lightly compressed cylinders become vastly more complex at high compressive strains or aspect ratios. We then exploit these landscapes to introduce an effective method for targeted design - landscape biasing. This is used to inform thickness modifications enabling landscape redesign, and the development of structures which are highly resistant to lateral perturbations. Our methods are general, and can be extended to studying postbuckling responses of other geometries.",1910.09210v1 2019-11-07,Long- to short-junction crossover and field-reentrant critical current in Al/Ag-nanowires/Al Josephson junctions,"We have probed the superconducting proximity effect through long high-quality monocrystalline Ag nanowires, by realizing Josephson junctions of different lengths, with different superconducting materials. Thanks to the high number of junctions probed, both the contact resistance and electron diffusion constant could be determined, enabling a comparison of the measured critical current to theoretical expectation, over the entire regime from short to long diffusive junction. Although the length dependence of the critical current is as expected, the amplitude of the $R_{N}I_c$ product is smaller than predicted by theory. We also address the magnetic field dependence of the critical current. The quasi-gaussian decay of the critical current with field expected of a long narrow junction is observed for all superconducting contacts we used except for aluminum. We present the striking non-monotonous effect of field on the critical current of junctions with aluminum contacts, and analyze it in terms of improved quasiparticle thermalization by a magnetic field.",1911.02962v1 2019-11-13,Giant enhancement of cryogenic thermopower by polar structural instability in the pressurized semimetal MoTe2,"We found that a high mobility semimetal 1T'-MoTe2 shows a significant pressure-dependent change in the cryogenic thermopower in the vicinity of the critical pressure, where the polar structural transition disappears. With the application of a high pressure of 0.75 GPa, while the resistivity becomes as low as 10 {\mu}{\Omega}cm, thermopower reached the maximum value of 60 {\mu}VK-1 at 25 K, leading to a giant thermoelectric power factor of 300 {\mu}WK-2cm-1. Based on semiquantitative analyses, the origin of this behavior is discussed in terms of inelastic electron-phonon scattering enhanced by the softening of zone center phonon modes associated with the polar structural instability.",1911.05269v1 2019-11-26,One-directional thermal transport in densely aligned single-wall carbon nanotube films,"Individual carbon nanotubes (CNTs) possess extremely high thermal conductivities. However, the thermal conductivities and their anisotropy of macroscopic assemblies of CNTs have so far remained small. Here, we report results of directional thermal transport measurements on a nearly-perfectly aligned CNT film fabricated via controlled vacuum filtration. We found the thermal conductivity to be 43 +- 2.2 W m^-1 K^-1 with a record-high thermal anisotropy of 500. From the temperature dependence of the thermal conductivity and its agreement with the atomistic phonon transport calculation, we conclude that the effect of intertube thermal resistance on heat conduction in the alignment direction is negligible because of the large contact area between CNTs. These observations thus represent ideal unidirectional thermal transport, i.e., the thermal conductivity of the film is determined solely by that of individual CNTs.",1911.11340v1 2020-05-05,Nanofilm Materials for Devices of Magnetic Field Measurement in Radiation Environment,"The prospects of using nanofilms of indium-containing III-V semiconductors, gold and single-layer graphene in magnetic field sensors, intended for application in radiation environment were evaluated on the results of testing in neutron fluxes. Semiconductor sensors are capable of withstanding radiation levels typical for the ITER-type fusion reactors, while gold sensors are stable even under environment expected in the first fusion power plant DEMO. Graphene is promising for creating sensors that combine high magnetic field sensitivity and high irradiation resistance.",2005.02075v1 2020-11-11,"Synthesis of high-entropy-alloy-type superconductors (Fe,Co,Ni,Rh,Ir)Zr2 with tunable transition temperature","We report on the synthesis and superconductivity of high-entropy-alloy-type (HEA-type) compounds TrZr2 (Tr = Fe, Co, Ni, Rh, Ir), in which the Tr site satisfies the criterion of HEA. Polycrystalline samples of HEA-type TrZr2 with four different compositions at the Tr site were synthesized by arc melting method. The phase purity and crystal structure were examined by Rietveld refinement of X-ray diffraction profile. It has been confirmed that the obtained samples have a CuAl2-type tetragonal structure. From analyses of elemental composition and mixing entropy at the Tr site, the HEA state for the Tr site was confirmed. The physical properties of obtained samples were characterized by electrical resistivity and magnetization measurements. All the samples show bulk superconductivity with various transition temperature (Tc). The Tc varied according to the compositions and showed correlations with the lattice constant c and Tr-Zr bond lengths. Introduction of an HEA site in TrZr2 is useful to achieve systematic tuning of Tc with a wide temperature range, which would be a merit for superconductivity application.",2011.05590v1 2020-11-20,Large Thermoelectric Power Factor in Whisker Crystals of Solid Solutions of the One-Dimensional Tellurides Ta4SiTe4 and Nb4SiTe4,"One-dimensional tellurides Ta4SiTe4 and Nb4SiTe4 were found to show high thermoelectric performance below room temperature. This study reported the synthesis and thermoelectric properties of whisker crystals of Ta4SiTe4-Nb4SiTe4 solid solutions and Mo- or Ti-doped (Ta0.5Nb0.5)4SiTe4. Thermoelectric power of the solid solutions systematically increased with increasing Ta content, while their electrical resistivity was unexpectedly small. Mo- and Ti-doped (Ta0.5Nb0.5)4SiTe4 showed n- and p-type thermoelectric properties with large power factors exceeding 40 microW cm-1 K-2, respectively. The fact that not only Ta4SiTe4 and Nb4SiTe4 but also their solid solutions showed high performance indicated that this system is a promising candidate for thermoelectric applications at low temperatures.",2011.10162v1 2020-12-11,Absence of superconductivity in topological metal ScInAu$_2$,"The Heusler compound ScInAu$_2$ was previously reported to have a superconducting ground state with a critical temperature of 3.0 K. Recent high throughput calculations have also predicted that the material harbors a topologically non-trivial band structure similar to that reported for beta-PdBi$_2$. In an effort to explore the interplay between the superconducting and topological properties properties, electrical resistance, magnetization, and x-ray diffraction measurements were performed on polycrystalline ScInAu$_2$. The data reveal that high-quality polycrystalline samples lack the super-conducting transition present samples that have not been annealed. These results indicate the earlier reported superconductivity is non-intrinsic. Several compounds in the Au-In-Sc ternary phase space (ScAu$_2$, ScIn$_3$, and ScInAu$_2$) were explored in an attempt to identify the secondary phase responsible for the non-intrinsic superconductivity. The results suggest that elemental In is responsible for the reported superconductivity in ScInAu$_2$.",2012.06501v1 2021-02-24,"Synthesis of new high-entropy alloy-type Nb3 (Al, Sn, Ge, Ga, Si) superconductors","Studies on high-entropy alloy (HEA) superconductors have recently been increasing, particularly in the fields of materials science and condensed matter physics. To contribute to research on new HEA-type superconductors, in our study we synthesized polycrystalline samples of A15-type superconductors of Nb3Al0.2Sn0.2Ge0.2Ga0.2Si0.2 (#1) and Nb3Al0.3Sn0.3Ge0.2Ga0.1Si0.1 (#2) with an HEA-type site by arc melting. Elemental and structural analyses revealed that the compositions of the obtained samples satisfied the HEA state criteria. Superconducting transitions were observed at 9.0 and 11.0 K for #1 and #2, respectively, in the temperature dependence of magnetization and electrical resistivity. Specific heat measurements revealed that the Sommerfeld coefficient, Debye temperature, and {\Delta}C/{\gamma}Tc for the obtained samples were close to those reported for conventional Nb3Sn family superconductors.",2102.12271v1 2021-02-24,Spin waves and high-frequency response in layered superconductors with helical magnetic structure,"We evaluate the spin-wave spectrum and dynamic susceptibility in a layered superconductors with helical interlayer magnetic structure. We especially focus on the structure in which the moments rotate 90$^{\circ}$ from layer to layer realized in the iron pnictide RbEuFe$_{4}$As$_{4}$. The spin-wave spectrum in superconductors is strongly renormalized due to the long-range electromagnetic interactions between the oscillating magnetic moments. This leads to strong enhancement of the frequency of the mode coupled with uniform field and this enhancement exists only within a narrow range of the c-axis wave vectors of the order of the inverse London penetration depth. The key feature of materials like RbEuFe$_{4}$As$_{4}$ is that this uniform mode corresponds to the maximum frequency of the spin-wave spectrum with respect to c-axis wave vector. As a consequence, the high-frequency surface resistance acquires a very distinct asymmetric feature spreading between the bare and renormalized frequencies. We also consider excitation of spin waves with Josephson effect in a tunneling contact between helical-magnetic and conventional superconductors and study the interplay between the spin-wave features and geometrical cavity resonances in the current-voltage characteristics.",2102.12445v2 2021-06-08,High electrical conduction of Sb square net in anti-ThCr$_2$Si$_2$ type La$_2$O$_2$Sb thin film grown by multilayer solid-phase epitaxy,"Anti-ThCr$_2$Si$_2$ type $RE_2$O$_2$Sb ($RE$ = rare earth) with Sb square net has shown insulating conduction so far. Here we report the synthesis of La$_2$O$_2$Sb epitaxial thin films for the first time by multilayer solid-phase epitaxy. The valence state of Sb was about -2 evaluated from X-ray photoemission spectroscopy measurement, and the indirect band gap of 0.17 eV was observed. The La$_2$O$_2$Sb epitaxial thin film showed unexpectedly high electrical conduction as a narrow gap semiconductor, whose resistivity at room temperature was approximately ten-thousand-fold lower than that of La$_2$O$_2$Sb bulk polycrystal, attributed to increased carrier mobility probably due to suppressed Sb dimerization.",2106.04713v1 2021-07-12,Hysteretic effects and magnetotransport of electrically switched CuMnAs,"Antiferromagnetic spintronics allows us to explore storing and processing information in magnetic crystals with vanishing magnetization. In this manuscript, we investigate magnetoresistance effects in antiferromagnetic CuMnAs upon switching into high-resistive states using electrical pulses. By employing magnetic field sweeps up to 14 T and magnetic field pulses up to $\sim$ 60 T, we reveal hysteretic phenomena and changes in the magnetoresistance, as well as the resilience of the switching signal in CuMnAs to the high magnetic field. These properties of the switched state are discussed in the context of recent studies of antiferromagnetic textures in CuMnAs.",2107.05724v1 2021-08-20,Quantum oscillations in an optically-illuminated two-dimensional electron system at the LaAlO$_3$/SrTiO$_3$ interface,"We have investigated the illumination effect on the magnetotransport properties of a two-dimensional electron system at the LaAlO$_3$/SrTiO$_3$ interface. The illumination significantly reduces the zero-field sheet resistance, eliminates the Kondo effect at low-temperature, and switches the negative magnetoresistance into the positive one. A large increase in the density of high-mobility carriers after illumination leads to quantum oscillations in the magnetoresistance originating from the Landau quantization. The carrier density ($\sim 2 \times 10^{12}$ cm$^{-2}$) and effective mass ($\sim 1.7 ~m_e$) estimated from the oscillations suggest that the high-mobility electrons occupy the d$_{xz/yz}$ subbands of Ti:t$_{2g}$ orbital extending deep within the conducting sheet of SrTiO$_3$. Our results demonstrate that the illumination which induces additional carriers at the interface can pave the way to control the Kondo-like scattering and study the quantum transport in the complex oxide heterostructures.",2108.09156v1 2021-11-27,Antiferromagnetic order in MnBi2Te4 films grown on Si(111) by molecular beam epitaxy,"MnBi2Te4 has recently been predicted and shown to be a magnetic topological insulator with intrinsic antiferromagnetic order. However, it remains a challenge to grow stoichiometric MnBi2Te4 films by molecular beam epitaxy (MBE) and to observe pure antiferromagnetic order by magnetometry. We report on a detailed study of MnBi2Te4 films grown on Si(111) by MBE with elemental sources. Films of about 100 nm thickness are analyzed in stoichiometric, structural, magnetic and magnetotransport properties with high accuracy. High-quality MnBi2Te4 films with nearly perfect septuple-layer structure are realized and structural defects typical for epitaxial van-der-Waals layers are analyzed. The films reveal antiferromagnetic order with a Neel temperature of 19 K, a spin-flop transition at a magnetic field of 2.5 T and a resistivity of 1.6 mOhm cm. These values are comparable to that of bulk MnBi2Te4 crystals. Our results provide an important basis for realizing and identifying single-phase MnBi2Te4 films with antiferromagnetic order grown by MBE.",2111.13960v1 2021-12-04,Superconducting and normal state properties of high entropy alloy Nb-Re-Hf-Zr-Tiinvestigated by muon spin relaxation and rotation,"Superconducting high entropy alloy (HEA) are emerging as a new class of superconducting materials. It provides a unique opportunity to understand the complex interplay of disorder and superconductivity. We report the synthesis and detail bulk and microscopic characterization of Nb$_{60}$Re$_{10}$Zr$_{10}$Hf$_{10}$Ti$_{10}$ HEA alloy using transport, magnetization, specific heat, and muon spin rotation/relaxation ($\mu$SR) measurements. Bulk superconductivity with transition temperature $T_{C}$ = 5.7 K confirmed by magnetization, resistivity, and heat capacity measurements. Zero-field $\mu$SR measurement shows that the superconducting state preserves time-reversal symmetry, and transverse-field measurements of the superfluid density are well described by an isotropic s-wave model.",2112.02388v1 2022-01-31,Disorder-mediated quenching of magnetization in NbVTiAl: Theory and Experiment,"In this paper, we present the structural, electronic, magnetic and transport properties of a equiatomic quaternary alloy NbVTiAl. The absence of (111) and (200) peaks in X-ray diffraction (XRD) data confirms the A2-type structure. Magnetization measurements indicate a high Curie temperature and a negligibly small magnetic moment ($\sim 10^{-3} \mu_B/f.u.$) These observations are indicative of fully compensated ferrimagnetism in the alloy. Temperature-dependent resistivity indicates metallic nature. Ab-initio calculation of fully ordered NbVTiAl structure confirms a nearly half metallic behavior with a high spin polarization ($\sim$ 90 \%) and a net magnetic moment of 0.8 $\mu_B/f.u.$ (in complete contrast to the experimental observation). One of the main objective of the present paper is to resolve and explain the long-standing discrepancy between theoretical prediction and experimental observation of magnetization for V-based quaternary Heusler alloys, in general. To gain an in-depth understanding, we modelled various disordered states and its subsequent effect on the magnetic and electronic properties. The discrepancy is attributed to the A2 disorder present in the system, as confirmed by our XRD data. The presence of disorder also causes the emergence of finite states at the Fermi level, which impacts the spin polarization of the system.",2201.13037v1 2022-03-12,Quantum transport evidence of the boundary states and Lifshitz transition in Bi$_4$Br$_4$,"The quasi-one-dimensional van der Waals compound Bi$_4$Br$_4$ was recently found to be a promising high-order topological insulator with exotic electronic states. In this paper, we study the electrical transport properties of Bi$_4$Br$_4$ bulk crystals. Two electron-type samples with different electron concentrations are investigated. Both samples have saturation resistivity behavior in low temperature. In the low-concentration sample, two-dimensional quantum oscillations are clearly observed in the magnetoresistance measurements, which are attributed to the band-bending-induced surface state on the (001) facet. In the high-concentration sample, the angular magnetoresistance exhibits two pairs of symmetrical sharp valleys with an angular difference close to the angle between the crystal planes (001) and (100). The additional valley can be explained by the contribution of the boundary states on the (100) facet. Besides, Hall measurements at low temperatures reveal an anomalous decrease of electron concentration with increasing temperature, which can be explained by the temperature-induced Lifshitz transition. These results shed light on the abundant surface and boundary state transport signals and the temperature-induced Lifshitz transition in Bi$_4$Br$_4$.",2203.06529v1 2022-06-21,Second harmonic AC calorimetry technique within a diamond anvil cell,"Tuning the energy density of matter at high pressures gives rise to exotic and often unprecedented properties, e.g., structural transitions, insulator-metal transitions, valence fluctuations, topological order, and the emergence of superconductivity. The study of specific heat has long been used to characterize these kinds of transitions, but their application to the diamond anvil cell (DAC) environment has proved challenging. Limited work has been done on the measurement of specific heat within DACs, in part due to the difficult experimental setup. To this end we have developed a novel method for the measurement of specific heat within a DAC that is independent of the DAC design and therefore readily compatible with any DACs already performing high pressure resistance measurements. As a proof-of-concept, specific heat measurements of the MgB2 superconductor were performed, showing a clear anomaly at the transition temperature (Tc), indicative of bulk superconductivity. This technique allows for specific heat measurements at higher pressure than previously possible.",2206.10072v1 2022-08-10,Synthesis and Superconductivity in Yttrium-Cerium Hydrides at Moderate Pressures,"Inspired by the high critical temperature in yttrium superhydride and the low stabilized pressure in superconducting cerium superhydride, we carry out four independent runs to synthesize yttrium-cerium alloy hydrides. The phases examined by the Raman scattering and x-ray diffraction measurements. The superconductivity is detected with the zero-resistance state at the critical temperature in the range of 97-140 K at pressures ranging from 114 GPa to 120$\pm$4 GPa. The maximum critical temperature of the synthesized hydrides is larger than those reported for cerium hydrides, while the corresponding stabilized pressure is much lower than those for superconducting yttrium hydrides. The structural analysis and theoretical calculations suggest that the phase of Y$_{0.5}$Ce$_{0.5}$H$_9$ has the space group $P6_3/mmc$ with the calculated critical temperature of 119 K, in fair agreement with the experiments. These results indicate that alloying superhydrides indeed can maintain relatively high critical temperature at modest pressures accessible by many laboratories.",2208.05191v1 2022-10-12,Field Induced Multiple Superconducting Phases in UTe2 along Hard Magnetic Axis,"The superconducting (SC) phase diagram in uranium ditelluride is explored under magnetic fields ($H$) along the hard magnetic b-axis using a high-quality single crystal with $T_{\rm c} = 2.1$ K. Simultaneous electrical resistivity and AC magnetic susceptibility measurements discern low- and high-field SC (LFSC and HFSC, respectively) phases with contrasting field-angular dependence. Crystal quality increases the upper critical field of the LFSC phase, but the $H^{\ast}$ of $\sim$15 T, at which the HFSC phase appears, is always the same through the various crystals. A phase boundary signature is also observed inside the LFSC phase near $H^{\ast}$, indicating an intermediate SC phase characterized by small flux pinning forces.",2210.05909v2 2022-10-20,Nanowire bolometer using a 2D high-temperature superconductor,"Superconducting nanowires are very important due to their applications ranging from quantum technology to astronomy. In this work, we implement a non-invasive process to fabricate nanowires of high-$T_\text{c}$ superconductor Bi$_2$Sr$_2$CaCu$_2$O$_{8+\delta}$ (BSCCO). We demonstrate that our nanowires can be used as bolometers in the visible range with very high responsivity of 9.7 $\times$ 10$^{3}$ V/W. Interestingly, in a long (30 $\mu$m) nanowire of 9 nm thickness and 700 nm width, we observe bias current-dependent localized spots of maximum photovoltage. Moreover, the scalability of the bolometer responsivity with the normal state resistance of the nanowire could allow further performance improvement by increasing the nanowire length in a meander geometry. We observe phase slip events in nanowires with small cross-sections (12 nm thick, 300 nm wide, and 3 $\mu$m long) at low temperatures. Our study presents a scalable method for realizing sensitive bolometers working near the liquid-nitrogen temperature.",2210.11254v2 2023-01-16,Role of disorder and strong 5$d$ electron correlation in the electronic structure of Sr2TiIrO6,"Transport and magnetic properties along with high resolution valence band photoemission study of disordered double perovskite Sr$_{2}$TiIrO$_{6}$ has been investigated. Insulator to insulator transition along with a magnetic transition concurrently occurs at 240 K. Comparison of valence band photoemission with band structure calculations suggests that the spin orbit coupling as well as electron correlation are necessary to capture the line shape and width of the Ir 5$d$ band. Room temperature valence band photoemission spectra show negligibly small intensity at Fermi energy, $E_{F}$. Fermi cut-off is observed at low temperatures employing high resolution. The spectral density of states at room temperature exhibits $|E-E_{F}|^{2}$ energy dependence signifying the role of electron-electron interaction. This energy dependence changes to $|E-E_{F}|^{3/2}$ below the magnetic transition evidencing the role of electron-magnon coupling in magnetically ordered state. The evolution of pseudogap ($\pm$12 meV) explains the sudden increase in resistivity ($\rho$) below 50 K in this disordered system. The temperature dependent spectral density of states at $E_{F}$ exhibiting $T^{1/2}$ behaviour verifies Altshuler-Aronov theory for correlated disordered systems.",2301.06275v1 2023-01-20,Giant resonant enhancement for photo-induced superconductivity in K$_3$C$_{60}$,"Photo-excitation at terahertz and mid-infrared frequencies has emerged as a new way to manipulate functionalities in quantum materials, in some cases creating non-equilibrium phases that have no equilibrium analogue. In K$_3$C$_{60}$, a metastable zero-resistance phase was documented with optical properties and pressure dependences compatible with non-equilibrium high temperature superconductivity. Here, we report the discovery of a dominant energy scale for this phenomenon, along with the demonstration of a giant increase in photo-susceptibility near 10 THz excitation frequency. At these drive frequencies a metastable superconducting-like phase is observed up to room temperature for fluences as low as ~400 $\mu J/cm^2$. These findings shed light on the microscopic mechanism underlying photo-induced superconductivity. They also trace a path towards steady state operation, currently limited by the availability of a suitable high-repetition rate optical source at these frequencies.",2301.08633v2 2023-02-13,Superconductivity with large upper critical field in noncentrosymmetric Cr-bearing high-entropy alloys,"A series of new Cr$_{5+x}$Mo$_{35-x}$W$_{12}$Re$_{35}$Ru$_{13}$C$_{20}$ high-entropy alloys (HEAs) have been synthesized and characterized by x-ray diffraction, scanning electron microscopy, electrical resistivity, magnetic susceptibility and specific heat measurements. It is found that the HEAs adopt a noncentrosymmetric cubic $\beta$-Mn type structure and exhibit bulk superconductivity for 0 $\leq$ $x$ $\leq$ 9. With increasing $x$, the cubic lattice parameter decreases from 6.7940(3) {\AA} to 6.7516(3) {\AA}. Meanwhile, the superconducting transition temperature $T_{\rm c}$ is suppressed from 5.49 K to 3.35 K due to the magnetic pair breaking caused by Cr moments. For all these noncentrosymmetric HEAs, the zero-temperature upper critical field $B_{\rm c2}$(0) is comparable to Pauli paramagnetic limit $B_{\rm P}$(0) = 1.86$T_{\rm c}$. In particular, the $B_{\rm c2}$(0)/$B_{\rm P}$(0) ratio reaches a maximum of $\sim$1.03 at $x$ = 6, which is among the highest for $\beta$-Mn type superconductors.",2302.06036v1 2023-02-23,Pressure induced electride phase formation in calcium: A key to its strange high-pressure behavior,"Elemental calcium (Ca), a simple metal at ambient conditions, has attracted huge interest because of its unusual high-pressure behavior in structural, electrical, and melting properties whose origin remain unsolved. Here, using a theoretical framework appropriate for describing electride phase formation, i.e., the presence of anionic electrons, we establish electride formation in Ca at a pressure as low as 8 GPa. Our analysis shows that under pressure the valence electrons of Ca localize at octahedral holes and exhibit anionic character which is responsible for its strange pressure behavior. Our calculated enthalpy and electrical resistance indicate that Ca will directly transform from an FCC-electride phase to an SC-electride phase near 30 GPa thereby avoiding the intermediate BCC phase. These findings are not limited to Ca but might hold a key to the understanding of host-guest type structures which occur in other elemental solids though at much higher pressures.",2302.11833v1 2023-05-16,Ambient and high-pressure electrical transport and structural investigations of magnetic Weyl semimetal PrAlGe,"We present ambient and high-pressure electrical transport and structural properties of recently discovered magnetic Weyl semimetal PrAlGe. Electrical resistivity at ambient pressure shows an anomaly at $T_C$ = 15.1 K related to the ferromagnetic transition. Anomalous Hall effect (AHE) is observed below $T_C$. We observe a 1.4 K/GPa increase of $T_C$ with pressure, resulting in $T_C$ $\approx$ 47 K at 23.0 GPa. Strong competition between Lorentz force and spin-scattering mechanisms suppressed by magnetic field is deduced from the magnetoresistance measurements under pressure. As in the ambient pressure case, the AHE is found to be present below $T_C$ up to the highest applied pressure. We observe a clear anomaly in the pressure dependence of $T_C$, magnetoresistance and Hall effect at 12.5 GPa suggesting the occurrence of a pressure-induced electronic transition at this pressure. X-ray diffraction (XRD) experiment under pressure revealed the lattice structure to be stable up to $\sim$19.6 GPa with the absence of any symmetry changing structural phase transition from the initial $I4_1md$ structure. Careful analysis of the pressure dependent XRD data reveal an isostructural transition near 11 GPa. Observed isostructural transition may be related to the pressure-induced electronic transition deduced from the magnetoresistance and Hall effect data.",2305.09298v1 2023-05-18,High-quality superconducting α-Ta film sputtered on heated silicon substrate,"Intrigued by the discovery of the long lifetime in the {\alpha}-Ta/Al2O3-based Transmon qubit, researchers recently found {\alpha}-Ta film is a promising platform for fabricating multi-qubits with long coherence time. To meet the requirements for integrating superconducting quantum circuits, the ideal method is to grow {\alpha}-Ta film on a silicon substrate compatible with industrial manufacturing. Here we report the {\alpha}-Ta film sputter-grown on Si (100) with a low-loss superconducting TiNx buffer layer. The {\alpha}-Ta film with a large growth temperature window has a good crystalline character. The superconducting critical transition temperature (Tc) and residual resistivity ratio (RRR) in the {\alpha}-Ta film grown at 500 {\deg}C are higher than that in the {\alpha}-Ta film grown at room temperature (RT). These results provide crucial experimental clues toward understanding the connection between the superconductivity and the materials' properties in the {\alpha}-Ta film and open a new route for producing a high-quality {\alpha}-Ta film on silicon substrate for future industrial superconducting quantum computers.",2305.10957v2 2023-05-20,A Computational Approach for Mapping Electrochemical Activity of Multi-Principal Element Alloys,"Multi principal element alloys (MPEAs) comprise a unique class of metal alloys. MPEAs have been demonstrated to possess several exceptional properties, including, as most relevant to the present study, a high corrosion resistance. In the context of MPEA design, the vast number of potential alloying elements and the staggering number of elemental combinations favours a computational alloy design approach. In order to computationally assess the prospective corrosion performance of MPEA, an approach was developed in this study. A density functional theory (DFT) based Monte Carlo method was used for the development of MPEA structure, with the AlCrTiV alloy used as a model. High-throughput DFT calculations were performed to create training datasets for surface activity towards different adsorbate species: O2-, Cl- and H+. Machine learning (ML) with combined representation was then utilised to predict the adsorption and vacancy energies as descriptors for surface activity. The capability of the combined computational methods of MC, DFT and ML, as a virtual electrochemical performance simulator for MPEAs was established and may be useful in exploring other MPEAs.",2305.12059v1 2023-06-16,Epitaxial α-Ta (110) film on a-plane sapphire substrate for superconducting qubits on wafer scale,"Realization of practical superconducting quantum computing requires many qubits of long coherence time. Compared to the commonly used Ta deposited on c-plane sapphire, which occasionally form {\alpha}-Ta (111) grains and \b{eta}-tantalum grains, high quality Ta (110) film can grow epitaxial on a-plane sapphire because of the atomic relationships at the interface. Well-ordered {\alpha}-Ta (110) film on wafer-scale a-plane sapphire has been prepared. The film exhibits high residual resistance ratio. Transmon qubits fabricated using these film shows relaxation times exceeding 150 {\mu}s. The results suggest Ta film on a-plane sapphire is a promising choice for long coherence time qubit on wafer scale.",2306.09568v2 2023-08-07,Modeling of electrochemical oxide film growth -- impact of band-to-band tunneling,"The Point Defect Model (PDM) describes the corrosion resistance properties of oxide films based on interfacial reactions and defect transport, which are affected by the electric field inside the oxide film. The PDM assumes a constant electric field strength due to band-to-band tunneling (BTBT) of electrons and the separation of electrons and holes by high electric fields. In this manuscript we present a more complex expansion of the common models to simulate steady state oxide films to test this assumption. The R-PDM was extended by including the transport of electrons and holes and BTBT. It could be shown that BTBT only occurs in very rare cases of narrow band gaps and high electric fields and the impact of electrons and holes does indeed lead to a buffering effect on the electric field, but does not lead to a constant electric field strength. Modeling the transport of electrons and holes on the oxide film allows to specifically estimate their potential impact on the film growth. Especially during modeling of oxide films with narrow band gap and/or electrochemical reactions at the film/solution interface the electrons and holes needs to be included to the model.",2308.05113v1 2023-09-09,High-throughput screening of coherent topologically close-packed precipitates in hexagonal close-packed metallic systems,"The nanoscale, coherent topologically close-packed (TCP) precipitate plates in magnesium alloys are found beneficial to the strength and creep resistance of alloys. However, the conventional trial-and-error method is too time-consuming and costly, which impedes the application of TCP precipitates to hcp-based metallic alloys. Here, we systematically screen the potential coherent TCP precipitate plates in the three most common hcp alloys, magnesium (Mg), titanium (Ti), and zirconium (Zr) alloys, using an efficient high-throughput screening methodology. Our findings indicate that the hcp-to-TCP structural transformations readily occur in Mg alloys, leading to abundant precipitation of TCP plates. However, hcp-Ti and Zr alloys exhibit a preference for hcp-to-bcc structural transformations, rather than the in situ precipitation of TCP plates. These screening results are largely consistent with experimental observations. The insights gained contribute to a deeper understanding of precipitation behavior in various hcp-based alloys at the atomic level and provide insightful reference results for designing novel alloys containing TCP phases.",2309.04822v2 2023-09-18,Superconductivity in the bcc-type High-entropy Alloy TiHfNbTaMo,"X-ray powder diffraction, electrical resistivity, magnetization, and thermodynamic measurements were conducted to investigate the structure and superconducting properties of TiHfNbTaMo, a novel high-entropy alloy possessing a valence electron count (VEC) of 4.8. The TiHfNbTaMo HEA was discovered to have a body-centered cubic structure and a microscopically homogeneous distribution of the constituent elements. This material shows type-II superconductivity with Tc = 3.42 K, lower critical field with 22.8 mT, and upper critical field with 3.95 T. Low-temperature specific heat measurements show that the alloy is a conventional s-wave type with a moderately coupled superconductor. First-principles calculations show that the density of states (DOS) of the TiHfNbTaMo alloy is dominated by hybrid d orbitals of these five metal elements. Additionally, the TiHfNbTaMo HEA exhibits three van Hove singularities. Furthermore, the VEC and the composition of the elements (especially the Nb elemental content) affect the Tc of the bcc-type HEA.",2309.09494v1 2023-11-26,On the special oxidation mechanism of a Mg-Y-Al alloy contained LPSO phase at high temperatures,"This work investigated the oxidation of Mg-11Y-1Al alloy in Ar-20%O2 at 500{\deg}through multiscale characterization. The results show that the network-like long-period stacking ordered(LPSO) phase decomposed into a needle-like LPSO phase and a polygonal Mg24Y5 phase. The needle-like LPSO phase resulted in the formation of a high-dense of needle-like oxide at the oxidation front of the area initially occupied by the network-like LPSO phase. The further inward oxygen would diffuse along the needle-like oxide-matrix interfaces and react with Y in the surrounding Mg matrix, resulting in the lateral growth of these needle-like oxides. Finally, the discrete needle-like oxides were interconnected to form a thicker and continuous oxide scale which could be more effective in hindering the elemental diffusion. Meanwhile, Al could partially enter the Y2O3 oxide scale and formed a strengthened (Y,Al)O oxide scale which could show a greater resistance to cracking and debonding.",2311.15182v1 2024-03-29,Metamagnetism in the high-pressure tetragonal phase of UTe$_2$,"A structural orthorhombic-to-tetragonal phase transition was recently discovered in the heavy-fermion compound UTe$_2$ at a pressure $p^*\simeq3-8$~GPa [Honda \textit{et al.}, J. Phys. Soc. Jpn. \textbf{92}, 044702 (2023); Huston \textit{et al.}, Phys. Rev. Mat. \textbf{6}, 114801 (2022)]. In the high-pressure tetragonal phase, a phase transition at $T_x=235$~K and a superconducting transition at $T_{sc}=2$~K have been revealed. In this work, we present an electrical-resistivity study of UTe$_2$ in pulsed magnetic fields up to $\mu_0H=58$~T combined with pressures up to $p$ = 6 GPa. The field was applied in a direction tilted by 30~$^\circ$~from \textbf{b} to \textbf{c} in the orthogonal structure, which is identified as the direction \textbf{c} of the tetragonal structure. In the tetragonal phase, the presence of superconductivity is confirmed and signatures of metamagnetic transitions are observed at the fields $\mu_0H_{x1}=24$~T and $\mu_0H_{x2}=34$~T and temperatures smaller than $T_x$. We discuss the effects of uniaxial pressure and we propose that a magnetic ordering drives the transition at $T_x$.",2403.20277v1 2024-04-17,Anisotropic Nonsaturating Magnetoresistance Observed in HoMn$_6$Ge$_6$: A Kagome Dirac Semimetal,"We report the magnetic and magnetotransport properties and electronic band structure of the kagome Dirac semimetal HoMn$_6$Ge$_6$. Temperature-dependent electrical resistivity demonstrates various magnetic-transition-driven anomalies. Notably, a crossover from negative to positive magnetoresistance (MR) is observed at around 150 K. While the linear nonsaturating positive MR in the low-temperature region is mainly driven by the linear Dirac-like band dispersions as predicted by the first-principles calculations, the negative MR observed in the high-temperature region is due to the spin-flop type magnetic transition. Consistent with anisotropic Fermi surface topology, we observe anisotropic magnetoresistance at low temperatures. A significant anomalous Hall effect has been noticed at high temperatures in addition to a switching of the dominant charge carrier from electron to hole at around 215 K.",2404.11414v2 2009-01-15,Metal-insulator transition and electroresistance in lanthanum/calcium manganites La_<1-x>Ca_MnO_<3> (x = 0-0.5) from voltage-current-temperature surfaces,"Of the perovskites, ABX_<3>, a subset of special interest is the family in which the A site is occupied by a lanthanide ion, the B site by a rare earth and X is oxygen, as such materials often exhibit a large change in electrical resistance in a magnetic field, a phenomenon known as ""colossal"" magnetoresistance (MR). Two additional phenomena in this family have also drawn attention: the metal-insulator transition (MIT) and electroresistance (ER). The MIT is revealed by measuring resistance as a function of temperature, and observing a change in the sign of the gradient. ER - the dependence of the resistance on applied current - is revealed by measuring resistance as a function of applied current. Up until now, the phenomena of MIT and ER have been treated separately. Here we report simultaneous observation of the MIT and ER in the lanthanum/calcium manganites. We accomplish this by measuring voltage-current curves over a wide temperature range (10-300 K) allowing us to build up an experimental voltage surface over current-temperature axes. These data directly lead to resistance surfaces. This approach provides additional insight into the phenomena of electrical transport in the lanthanum/calcium manganites, in particular the close connection of the maximum ER to the occurrence of the MIT in those cases of a paramagnetic insulator (PMI) to ferromagnetic metal (FMM) transition.",0901.2243v1 2009-10-24,Monte Carlo Study of the Spin Transport in Magnetic Materials,"The resistivity in magnetic materials has been theoretically shown to depend on the spin-spin correlation function which in turn depends on the magnetic-field, the density of conduction electron, the magnetic ordering stability, etc. However, these theories involved a lot of approximations, so their validity remained to be confirmed. The purpose of this work is to show by extensive Monte Carlo (MC) simulation the resistivity of the spin current from low-$T$ ordered phase to high-$T$ paramagnetic phase in a ferromagnetic film. We take into account the interaction between the itinerant spins and the localized lattice spins as well as the interaction between itinerant spins themselves. We show that the resistivity undergoes an anomalous behavior at the magnetic phase transition in agreement with previous theories in spite of their numerous approximations. The origin of the resistivity peak near the phase transition in ferromagnets is interpreted here as stemming from the existence of magnetic domains in the critical region. This interpretation is shown to be in consistence with previous theoretical pictures. Resistivity in a simple cubic antiferromagnet is also shown. The absence of a peak in this case is explained.",0910.4619v3 2021-01-04,Thermal Resistance at a Twist Boundary and Semicoherent Heterointerface,"Traditional models of interfacial phonon scattering, including the acoustic mismatch model (AMM) and diffuse mismatch model (DMM), take into account the bulk properties of the material surrounding the interface, but not the atomic structure and properties of the interface itself. Here, we derive a theoretical formalism for the phonon scattering at a dislocation grid, or two interpenetrating orthogonal arrays of dislocations, as this is the most stable structure of both the symmetric twist boundary and semicoherent heterointerface. With this approach, we are able to separately examine the contribution to thermal resistance due to the step function change in acoustic properties and due to interfacial dislocation strain fields, which induces diffractive scattering. Both low-angle Si-Si twist boundaries and the Si-Ge heterointerfaces are considered here and compared to previous experimental and simulation results. This work indicates that scattering from misfit dislocation strain fields doubles the thermal boundary resistance of Si-Ge heterointerfaces compared to scattering due to acoustic mismatch alone. Scattering from grain boundary dislocation strain fields is predicted to dominate the thermal boundary resistance of Si-Si twist boundaries. This physical treatment can guide the thermal design of devices by quantifying the relative importance of interfacial strain fields, which can be engineered via fabrication and processing methods, versus acoustic mismatch, which is fixed for a given interface. Additionally, this approach captures experimental and simulation trends such as the dependence of thermal boundary resistance on the grain boundary angle and interfacial strain energy.",2101.01058v2 2015-07-15,Influence of Periodic Surface Nanopatterning Profiles on Series Resistance in Thin-Film Crystalline Silicon Heterojunction Solar Cells,"In the frame of the development of thin crystalline silicon solar cell technologies, surface nanopatterning of silicon is gaining importance. Its impact on the material quality is, however, not yet fully controlled.We investigate here the influence of surface nanotexturing on the series resistance of a contacting scheme relevant for thin-film crystalline silicon heterojunction solar cells. Two dimensional periodic nanotextures are fabricated using a combination of nanoimprint lithography and either dry or wet etching, while random pyramid texturing is used for benchmarking. We compare these texturing techniques in terms of their effect on the series resistance of a solar cell through a study of the sheet resistance (Rsh ) and contact resistance (Rc) of its front layers, i.e., a sputtered transparent conductive oxide and evaporated metal contacts. We have found by four-point probe and the transfer length methods that dry-etched nanopatterns render the highest Rsh and Rc values. Wet-etched nanopatterns, on the other hand, have less impact on Rc and render Rsh similar to that obtained from the nontextured case.",1507.07819v1 2023-01-12,On the switching mechanism and optimisation of ion irradiation enabled 2D $MoS_2$ memristors,"Memristors are prominent passive circuit elements with promising futures for energy-efficient in-memory processing and revolutionary neuromorphic computation. State-of-the-art memristors based on two-dimensional (2D) materials exhibit enhanced tunability, scalability and electrical reliability. However, the fundamental of the switching is yet to be clarified before they can meet industrial standards in terms of endurance, variability, resistance ratio, and scalability. This new physical simulator based on the kinetic Monte Carlo (kMC) algorithm reproduces the defect migration process in 2D materials and sheds light on the operation of 2D memristors. The present work employs the simulator to study a two-dimensional $2H-MoS_2$ planar resistive switching (RS) device with an asymmetric defect concentration introduced by ion irradiation. The simulations unveil the non-filamentary RS process and propose practical routes to optimize the device's performance. For instance, the resistance ratio can be increased by 53% by controlling the concentration and distribution of defects, while the variability can be reduced by 55% by increasing 5-fold the device size from 10 to 50 nm. Our simulator also explains the trade-offs between the resistance ratio and variability, resistance ratio and scalability, and variability and scalability. Overall, the simulator may enable an understanding and optimization of devices to expedite cutting-edge applications.",2301.05260v2 2011-12-13,Online in-situ X-ray diffraction setup for structural modification studies during swift heavy ion irradiation,"The high energy density of electronic excitations due to the impact of swift heavy ions can induce structural modifications in materials. We present a X-ray diffractometer called ALIX, which has been set up at the low-energy IRRSUD beamline of the GANIL facility, to allow the study of structural modification kinetics as a function of the ion fluence. The X-ray setup has been modified and optimized to enable irradiation by swift heavy ions simultaneously to X-ray pattern recording. We present the capability of ALIX to perform simultaneous irradiation - diffraction by using energy discrimination between X-rays from diffraction and from ion-target interaction. To illustrate its potential, results of sequential or simultaneous irradiation - diffraction are presented in this article to show radiation effects on the structural properties of ceramics. Phase transition kinetics have been studied during xenon ion irradiation of polycrystalline MgO and SrTiO3. We have observed that MgO oxide is radiation-resistant to high electronic excitations, contrary to the high sensitivity of SrTiO3, which exhibits transition from the crystalline to the amorphous state during irradiation. By interpreting the amorphization kinetics of SrTiO3, defect overlapping models are discussed as well as latent track characteristics. Together with a transmission electron microscopy study, we conclude that a single impact model describes the phase transition mechanism.",1112.2832v2 2017-10-07,High pressure x-ray study of spin-Peierls physics in the quantum spin chain material TiOCl,"The application of pressure can induce transitions between unconventional quantum phases in correlated materials. The inorganic compound TiOCl, composed of chains of S=1/2 Ti ions, is an ideal realization of a spin-Peierls system with a relatively simple unit cell. At ambient pressure, it is an insulator due to strong electronic interactions (a Mott insulator). Its resistivity shows a sudden decrease with increasing pressure, indicating a transition to a more metallic state which may coincide with the emergence of charge density wave order. Therefore, high pressure studies of the structure with x-rays are crucial in determining the ground-state physics in this quantum magnet. In ambient pressure, TiOCl exhibits a transition to an incommensurate nearly dimerized state at $T_{c2}=92$ K and to a commensurate dimerized state at $T_{c1}=66$ K. Here, we discover a rich phase diagram as a function of temperature and pressure using x-ray diffraction on a single crystal in a diamond anvil cell down to $T=4$ K and pressures up to 14.5 GPa. Remarkably, the magnetic interaction scale increases dramatically with increasing pressure, as indicated by the high onset temperature of the spin-Peierls phase. At $\sim$7 GPa, the extrapolated onset of the spin-Peierls phase occurs above $T=300$ K, indicating a quantum singlet state exists at room temperature. Further comparisons are made with the phase diagrams of related spin-Peierls systems that display metallicity and superconductivity under pressure.",1710.02632v1 2019-02-28,Quenched nematic criticality separating two superconducting domes in an iron-based superconductor under pressure,"The nematic electronic state and its associated nematic critical fluctuations have emerged as potential candidates for superconducting pairing in various unconventional superconductors. However, in most materials their coexistence with other magnetically-ordered phases poses significant challenges in establishing their importance. Here, by combining chemical and hydrostatic physical pressure in FeSe$_{0.89}$S$_{0.11}$, we provide a unique access to a clean nematic quantum phase transition in the absence of a long-range magnetic order. We find that in the proximity of the nematic phase transition, there is an unusual non-Fermi liquid behavior in resistivity at high temperatures that evolves into a Fermi liquid behaviour at the lowest temperatures. From quantum oscillations in high magnetic fields, we trace the evolution of the Fermi surface and electronic correlations as a function of applied pressure. We detect experimentally a Lifshitz transition that separates two distinct superconducting regions: one emerging from the nematic electronic phase with a small Fermi surface and strong electronic correlations and the other one with a large Fermi surface and weak correlations that promotes nesting and stabilization of a magnetically-ordered phase at high pressures. The lack of mass divergence suggests that the nematic critical fluctuations are quenched by the strong coupling to the lattice. This establishes that superconductivity is not enhanced at the nematic quantum phase transition in the absence of magnetic order.",1902.11276v1 2020-09-03,Topological Nature of High Temperature Superconductivity,"The key to unraveling the nature of high-temperature superconductivity (HTS) lies in resolving the enigma of the pseudogap state. The pseudogap state in the underdoped region is a distinct thermodynamic phase characterized by nematicity, temperature-quadratic resistive behavior, and magnetoelectric effects. Till present, a general description of the observed universal features of the pseudogap phase and their connection with HTS was lacking. The proposed work constructs a unifying effective field theory capturing all universal characteristics of HTS materials and explaining the observed phase diagram. The pseudogap state is established to be a phase where a charged magnetic monopole condensate confines Cooper pairs to form an oblique version of a superinsulator. The HTS phase diagram is dominated by a tricritical point (TCP) at which the first order transition between a fundamental Cooper pair condensate and a charged magnetic monopole condensate merges with the continuous superconductor-normal metal and superconductor-pseudogap state phase transitions. The universality of the HTS phase diagram reflects a unique topological mechanism of competition between the magnetic monopole condensate, inherent to antiferromagnetic-order-induced Mott insulators and the Cooper pair condensate. The obtained results establish the topological nature of the HTS and provide a platform for devising materials with the enhanced superconducting transition temperature.",2009.01763v2 2020-09-16,Tailoring c-axis orientation in epitaxial Ruddlesden-Popper Pr$_{0.5}$Ca$_{1.5}$MnO$_{4}$ films,"Interest for layered Ruddlesden-Popper strongly correlated manganites of Pr$_{0.5}$Ca$_{1.5}$MnO$_4$ as well as to their thin film polymorphs is motivated by the high temperature of charge orbital ordering above room temperature. We report on the tailoring of the c-axis orientation in epitaxial RP-PCMO films grown on SrTiO$_3$ (STO) substrates with different orientations as well as the use of CaMnO$_3$ (CMO) buffer layers. Films on STO(110) reveal in-plane alignment of the c-axis lying along to the [100] direction. On STO(100), two possible directions of the in-plane c-axis lead to a mosaic like, quasi two-dimensional nanostructure, consisting of RP, rock-salt and perovskite building blocks. With the use of a CMO buffer layer, RP-PCMO epitaxial films with c-axis out-of-plane were realized. Different physical vapor deposition techniques, i.e. ion beam sputtering (IBS), pulsed laser deposition (PLD) as well as metalorganic aerosol deposition (MAD) are applied in order to distinguish between the effect of growth conditions and intrinsic epitaxial properties. For all deposition techniques, despite their very different growth conditions, the surface morphology, crystal structure and orientation of the thin films reveal a high level of similarity as verified by X-ray diffraction, scanning and high resolution transmission electron microscopy. We found that for different epitaxial relations the stress in the films can be relaxed by means of a modified interface chemistry. The charge ordering in the films estimated by resistivity measurements occurs at a temperature close to that expected in bulk material.",2009.07523v1 2020-09-28,Pressure-induced reconstructive phase transition in Cd$_3$As$_2$,"Cadmium arsenide Cd$_3$As$_2$ hosts massless Dirac electrons in its ambient-conditions tetragonal phase. We report X-ray diffraction and electrical resistivity measurements of Cd$_3$As$_2$ upon cycling pressure beyond the critical pressure of the tetragonal phase and back to ambient conditions. We find that at room temperature the transition between the low- and high-pressure phases results in large microstrain and reduced crystallite size both on rising and falling pressure. This leads to non-reversible electronic properties including self-doping associated with defects and a reduction of the electron mobility by an order of magnitude due to increased scattering. Our study indicates that the structural transformation is sluggish and shows a sizable hysteresis of over 1~GPa. Therefore, we conclude that the transition is first-order reconstructive, with chemical bonds being broken and rearranged in the high-pressure phase. Using the diffraction measurements we demonstrate that annealing at ~200$^\circ$C greatly improves the crystallinity of the high-pressure phase. We show that its Bragg peaks can be indexed as a primitive orthorhombic lattice with a_HP~8.68 A b_HP~17.15 A and c_HP~18.58 A. The diffraction study indicates that during the structural transformation a new phase with another primitive orthorhombic structure may be also stabilized by deviatoric stress, providing an additional venue for tuning the unconventional electronic states in Cd3As2.",2009.13228v2 2016-03-01,Superconductivity in HfTe5 Induced via Pressures,"Recently, ZrTe5 and HfTe5 are theoretically studied to be the most promising layered topological insulators since they are both interlayer weakly bonded materials and also with a large bulk gap in the single layer. It paves a new way for the study of novel topological quantum phenomenon tuned via external parameters. Here, we report the discovery of superconductivity and properties evolution in HfTe5 single crystal induced via pressures. Our experiments indicated that anomaly resistance peak moves to low temperature first before reverses to high temperature followed by disappearance which is opposite to the low pressure effect on ZrTe5. HfTe5 became superconductive above ~5.5 GPa up to at least 35 GPa in the measured range. The highest superconducting transition temperature (Tc) around 5 K was achieved at 20 GPa. High pressure Raman revealed that new modes appeared around pressure where superconductivity occurs. Crystal structure studies shown that the superconductivity is related to the phase transition from Cmcm structure to monoclinic C2/m structure. The second phase transition from C2/m to P-1 structure occurs at 12 GPa. The combination of transport, structure measurement and theoretical calculations enable a completely phase diagram of HfTe5 at high pressures.",1603.00514v1 2021-01-29,Tunable Doping of Rhenium and Vanadium into Transition Metal Dichalcogenides for Two-Dimensional Electronics,"Two-dimensional (2D) transition metal dichalcogenides (TMDCs) with unique electrical properties are fascinating materials used for future electronics. However, the strong Fermi level pinning effect at the interface of TMDCs and metal electrodes always leads to high contact resistance, which seriously hinders their application in 2D electronics. One effective way to overcome this is to use metallic TMDCs or transferred metal electrodes as van der Waals (vdW) contacts. Alternatively, using highly conductive doped TMDCs will have a profound impact on the contact engineering of 2D electronics. Here, a novel chemical vapor deposition using mixed molten salts is established for vapor-liquid-solid growth of high-quality rhenium (Re) and vanadium (V)-doped TMDC monolayers with high controllability and reproducibility. A tunable semiconductor to metal transition is observed in the Re and V-doped TMDCs. Electrical conductivity increases up to a factor of 108 in the degenerate V-doped WS2 and WSe2. Using V-doped WSe2 as vdW contact, the on-state current and on/off ratio of WSe2-based field-effect transistors have been substantially improved (from ~10-8 to 10-5 A; ~104 to 108), compared to metal contacts. Future studies on lateral contacts and interconnects using doped TMDCs will pave the way for 2D integrated circuits and flexible electronics.",2101.12423v1 2020-11-05,Temperature-dependent elastic properties of binary and multicomponent high-entropy refractory carbides,"Available information concerning the elastic moduli of refractory carbides at temperatures (T) of relevance for practical applications is sparse and/or inconsistent. We carry out ab initio molecular dynamics (AIMD) simulations at T = 300, 600, 900, and 1200 K to determine the temperature-dependences of the elastic constants of rocksalt-structure (B1) TiC, ZrC, HfC, VC, and TaC compounds as well as multicomponent high-entropy carbides (Ti,Zr,Hf,Ta,W)C and (V,Nb,Ta,Mo,W)C. The second order elastic constants are calculated by least-square fitting of the analytical expressions of stress vs. strain relationships to simulation results obtained from three tensile and three shear deformation modes. Moreover, we employ sound velocity measurements to evaluate the bulk, shear, elastic moduli and Poisson's ratios of single-phase B1 (Ti,Zr,Hf,Ta,W)C and (V,Nb,Ta,Mo,W)C at ambient conditions. Our experimental results are in excellent agreement with the values obtained by AIMD simulations. In comparison with the predictions of previous ab initio calculations - where the extrapolation of finite-temperature elastic properties accounted for thermal expansion while neglecting intrinsic vibrational effects - AIMD simulations produce a softening of elastic moduli with T in closer agreement with experiments. Results of our simulations show that TaC is the system which exhibits the highest elastic resistances to both tensile and shear deformation up to 1200 K, and identify the high-entropy (V,Nb,Ta,Mo,W)C system as candidate for applications that require good ductility and toughness at room as well as elevated temperatures.",2011.02742v1 2021-03-09,Crack-free caustic magnesia-bonded refractory castables,"A growing interest in designing high-alumina MgO-bonded refractory castables has been identified in recent years due to the magnesia ability to react: (i) with water at the initial processing stages of these materials (inducing the precipitation of brucite phase) or (ii) with alumina, giving rise to in situ MgAl2O4 generation at high temperatures. Nevertheless, despite the great potential of caustic magnesia to be used as a binder in such systems due to its high reactivity, it is still a challenge to control the hydration reaction rate of this oxide and the negative effects derived from the expansive feature of Mg(OH)2 formation. Thus, this work evaluated the incorporation of different contents of aluminum hydroxyl lactate (AHL) into caustic magnesia-bonded castables, aiming to control the brucite precipitation during the curing and drying steps of the prepared samples, resulting in crack-free refractories. The designed compositions were characterized via flowability, setting behavior, X-ray diffraction, cold flexural strength, porosity, permeability and thermogravimetric measurements. According to the results, instead of Mg(OH)2, hydrotalcite-like phases [Mg6Al2(OH)16(OH)2.4.5H2O and Mg6Al2(OH)16(CO3).4H2O] were the main hydrated phases identified in the AHL-containing compositions. The addition of 1.0 wt.% of aluminum hydroxyl lactate to the designed castable proved to be, so far, the best option for this magnesia source, resulting in the development of a crack-free refractory with enhanced properties and greater spalling resistance under heating.",2103.05361v1 2021-03-20,Towards Superior High Temperature Properties in Low Density AlCrFeNiTi Compositionally Complex Alloys,"Three novel precipitation strengthened bcc alloys which exhibit a smooth microstructural gradient with composition have been fabricated in bulk form by induction casting. All three alloys are comprised of a mixture of disordered A2-(Fe, Cr) and L2$_1$-ordered (Ni, Fe)$_{2}$AlTi type phases both as-cast and after long-term annealing at 900 $^{\circ}$C. The ratio of disordered to ordered phase, primary dendrite fraction, and overall microstructural coarseness all decrease as Cr is replaced by Al and Ti. Differences in phase composition are quantified through domain averaged principal component analysis of energy dispersive spectroscopy data obtained during scanning transmission electron microscopy. Bulk tensile testing reveals retained strengths of nearly 250 MPa up to 900 $^{\circ}$C for the alloys which contain a nanoscale maze-like arrangement of ordered and disordered phases. One alloy, containing a duplex microstructure with ductile dendritic regions and highly creep resistant interdendritic regions, shows a promising balance between high temperature ductility and strength. For this alloy, tension creep testing was carried out at 700, 750, and 800 $^{\circ}$C for a broad range of loading conditions and revealed upper bound creep rates which surpass similar ferritic superalloys and rival those of several conventionally employed high temperature structural alloys, including Inconel 617 and 718, at much lower density and raw material cost.",2103.11173v1 2021-06-02,Dopant redistribution and activation in Ga ion-implanted high Ge content SiGe by explosive crystallization during UV nanosecond pulsed laser annealing,"Explosive crystallization (EC) is often observed when using nanosecond-pulsed melt laser annealing (MLA) in amorphous silicon (Si) and germanium (Ge). The solidification velocity in EC is so fast that a diffusion-less crystallization can be expected. In the contacts of advanced transistors, the active level at the metal/semiconductor Schottky interface must be very high to achieve a sub-10^{-9} ohm.cm2 contact resistivity, which has been already demonstrated by using the dopant surface segregation induced by MLA. However, the beneficial layer of a few nanometers at the surface may be easily consumed during subsequent contact cleaning and metallization. EC helps to address such kind of process integration issues, enabling the optimal positioning of the peak of the dopant chemical profile. However, there is a lack of experimental studies of EC in heavily-doped semiconductor materials. Furthermore, to the best of our knowledge, dopant activation by EC has never been experimentally reported. In this paper, we present dopant redistribution and activation by an EC process induced by UV nanosecond-pulsed MLA in heavily gallium (Ga) ion-implanted high Ge content SiGe. Based on the obtained results, we also highlight potential issues of integrating EC into real device fabrication processes and discuss how to manage them.",2106.00946v1 2022-06-29,Designing wake-up free ferroelectric capacitors based on the $\mathrm{HfO_2/ZrO_2}$ superlattice structure,"The wake-up phenomenon widely exists in hafnia-based ferroelectric capacitors, which causes device parameter variation over time. Crystallization at higher temperatures have been reported to be effective in eliminating wake-up, but high temperature may yield the monoclinic phase or generate high concentration oxygen vacancies. In this work, a unidirectional annealing method is proposed for the crystallization of $\mathrm{Hf_{0.5}Zr_{0.5}O_2}$ (HZO) superlattice ferroelectrics, which involves heating from the $\mathrm{Pt/ZrO_2}$ interface side. Nanoscale $\mathrm{ZrO_2}$ is selected to resist the formation of monoclinic phase, and the chemically inert Pt electrode can avoid the continuous generation of oxygen vacancies during annealing. It is demonstrated that $\mathrm{600^oC}$ annealing only leads to a moderate content of monoclinic phase in HZO, and the TiN/HZO/Pt capacitor exhibits wake-up free nature and a $2P_\mathrm{r}$ value of 27.4 $\mu\mathrm{C/cm^2}$. On the other hand, heating from the $\mathrm{TiN/HfO_2}$ side, or using $\mathrm{500^oC}$ annealing temperature, both yield ferroelectric devices that require a wake-up process. The special configuration of $\mathrm{Pt/ZrO_2}$ is verified by comparative studies with several other superlattice structures and HZO solid-state solutions. It is discovered that heating from the $\mathrm{Pt/HfO_2}$ side at $\mathrm{600^oC}$ leads to high leakage current and a memristor behavior. The mechanisms of ferroelectric phase stabilization and memristor formation have been discussed. The unidirectional heating method can also be useful for other hafnia-based ferroelectric devices.",2206.14393v1 2022-09-06,Silicide-based Josephson field effect transistors for superconducting qubits,"Scalability in the fabrication and operation of quantum computers is key to move beyond the NISQ era. So far, superconducting transmon qubits based on aluminum Josephson tunnel junctions have demonstrated the most advanced results, though this technology is difficult to implement with large-scale facilities. An alternative ""gatemon"" qubit has recently appeared, which uses hybrid superconducting/semiconducting (S/Sm) devices as gate-tuned Josephson junctions. Current implementations of these use nanowires however, of which the large-scale fabrication has not yet matured either. A scalable gatemon design could be made with CMOS Josephson Field-Effect Transistors as tunable weak link, where an ideal device has leads with a large superconducting gap that contact a short channel through high-transparency interfaces. High transparency, or low contact resistance, is achieved in the microelectronics industry with silicides, of which some turn out to be superconducting. The first part of the experimental work in this thesis covers material studies on two such materials: $\text{V}_3\text{Si}$ and PtSi, which are interesting for their high $T_\text{c}$, and mature integration, respectively. The second part covers experimental results on 50 nm gate length PtSi transistors, where the transparency of the S/Sm interfaces is modulated by the gate voltage. At low voltages, the transport shows no conductance at low energy, and well-defined features at the superconducting gap. The barrier height at the S/Sm interface is reduced by increasing the gate voltage, until a zero-bias peak appears around zero drain voltage, which reveals the appearance of an Andreev current. The successful gate modulation of Andreev current in a silicon-based transistor represents a step towards fully CMOS-integrated superconducting quantum computers.",2209.02721v1 2023-03-21,Thermal decoupling in high-$T_c$ cuprate superconductors,"Although many years have passed since the discovery of high-critical-temperature (high-$T_c$) superconducting materials, the underlying mechanism is still unknown. The B1g phonon anomaly in high-Tc cuprate superconductors has long been studied; however, the correlation between the B1g phonon anomaly and superconductivity has yet to be clarified. In the present study, we successfully reproduced the B1g phonon anomaly in YBa$_2$Cu$_3$O$_7$ (YBCO) using an ab initio molecular dynamics (AIMD) simulation and temperature-dependent effective potential (TDEP) method. The Ag phonon by Ba atoms shows a more severe anomaly than the B1g phonon at low temperatures. Our analysis of the phonon anomaly and the temperature-dependent phonon dispersion indicated that decoupling between thermal phenomena and electron transport at low temperatures leads to layer-by-layer thermal decoupling in YBCO. Electronically and thermally isolated Ba atoms in YBCO are responsible for the thermal decoupling. The analytic study of the thermal dcoupling revealed that Planckian dissipation expressing linear-T resistivity is another expression of the Fermi liquid of the CuO$_2$ plane. The Uemura plot of the relationship between Tc and the Fermi temperature, as well as the superconducting dome in YBCO, is explained rigorously and quantitatively. Our findings not only present a new paradigm for understanding high-Tc superconductivity but also imply that the spontaneous formation of low-temperature layers in materials can lead to revolutionary changes in the thermal issues of industrial fields.",2303.11600v1 2023-03-24,A review on the advancements in the characterization of the high-pressure properties of iodates,"The goal of this work is to report a systematic and balanced review of the progress made in recent years on the high-pressure behavior of iodates, a group of materials with multiple technological applications and peculiar behaviors under external compression. This review article presents results obtained from multiple characterization techniques which include: X-ray diffraction, Raman and infrared spectroscopy, optical-absorption, resistivity, and second-harmonic generation measurements. The discussion of the results from experiments will be combined with density-functional theory calculations which have been shown to be a very useful tool for the interpretation of experimental data. Throughout the manuscript many of the phenomena observed will be connected to the presence of a lone electron pairs of the iodine atoms in the studied iodates. The presence of the lone electron pairs plays a crucial role in the high-pressure behavior of iodates and it is associated with many of the phenomena discussed here, in particular with the pressure-induced changes in the character of iodine-oxygen bonds, which causes many physical properties to behave nonlinearly. Towards the end of this review, a discussion of current problems that remain unsolved is presented as well as proposals for possible avenues for future studies.",2303.14215v1 2023-11-22,"Durable, ultrathin, and antifouling polymer brush coating for efficient condensation heat transfer","Heat exchangers are made of metals because of their high heat conductivity and mechanical stability. Metal surfaces are inherently hydrophilic, leading to inefficient filmwise condensation. It is still a challenge to coat these metal surfaces with a durable, robust and thin hydrophobic layer, which is required for efficient dropwise condensation. Here, we report the non-structured and ultrathin (~6 nm) polydimethylsiloxane (PDMS) brushes on copper that sustain high-performing dropwise condensation in high supersaturation. Due to the flexible hydrophobic siloxane polymer chains, the coating has low resistance to drop sliding and excellent chemical stability. The PDMS brushes can sustain dropwise condensation for up to ~8 h during exposure to 111 {\deg}C saturated steam flowing at 3 m/s, with a 5-7 times higher heat transfer coefficient compared to filmwise condensation. The surface is self-cleaning and can reduce bacterial attachment by 99%. This low-cost, facile, fluorine-free, and scalable method is suitable for a great variety of condensation heat transfer applications.",2311.13353v1 2023-12-01,"Insulator to Metal Transition, Spin-Phonon Coupling, and Potential Magnetic Transition Observed in Quantum Spin Liquid Candidate LiYbSe$_2$ under High Pressure","Metallization of quantum spin liquid (QSL) materials has long been considered as a potential route to achieve unconventional superconductivity. Here we report our endeavor in this direction by pressurizing a three-dimensional QSL candidate, LiYbSe$_2$, with a previously unreported pyrochlore structure. High-pressure X-ray diffraction and Raman studies up to 50 GPa reveal no appreciable changes of structural symmetry or distortion in this pressure range. This compound is so insulating that its resistance decreases below 10$^5$ ${\Omega}$ only at pressures above 25 GPa in the corresponding temperature range accompanying the gradual reduction of band gap upon compression. Interestingly, an insulator-to-metal transition takes place in LiYbSe$_2$ at about 68 GPa and the metallic behavior remains up to 123.5 GPa, the highest pressure reached in the present study. A possible sign of magnetic or other phase transition was observed in LiYbSe$_2$. The insulator-to-metal transition in LiYbSe$_2$ under high pressure makes it an ideal system to study the pressure effects on QSL candidates of spin-1/2 Yb$^{3+}$ system in different lattice patterns.",2312.00270v2 2024-01-06,Endless Dirac nodal lines and high mobility in kagome semimetal Ni3In2Se2 single crystal,"Kagome-lattice crystal is crucial in quantum materials research, exhibiting unique transport properties due to its rich band structure and the presence of nodal lines and rings. Here, we investigate the electronic transport properties and perform first-principles calculations for Ni$_{3}$In$_{2}$Se$_{2}$ kagome topological semimetal. First-principle calculations indicate six endless Dirac nodal lines and two nodal rings with a $\pi$-Berry phase in the Ni$_{3}$In$_{2}$Se$_{2}$ compound. The temperature-dependent resistivity is dominated by two scattering mechanisms: $s$-$d$ interband scattering occurs below 50 K, while electron-phonon ($e$-$p$) scattering is observed above 50 K. The magnetoresistance (MR) curve aligns with the theory of extended Kohler's rule, suggesting multiple scattering origins and temperature-dependent carrier densities. A maximum MR of 120\% at 2 K and 9 T, with a maximum estimated mobility of approximately 3000 cm$^{2}$V$^{-1}$s$^{-1}$ are observed. The Ni atom's hole-like d$_{x^{2}-y^{2} }$ and electron-like d$_{z^{2}}$ orbitals exhibit peaks and valleys, forming a local indirect-type band gap near the Fermi level (E$_{F}$). This configuration enhances the motion of electrons and holes, resulting in high mobility and relatively high magnetoresistance.",2401.03130v1 2024-04-18,Omnidirectional 3D printing of PEDOT:PSS aerogels with tunable electromechanical performance for unconventional stretchable interconnects and thermoelectrics,"The next generation of soft electronics will expand to the third dimension. This will require the integration of mechanically-compliant three-dimensional functional structures with stretchable materials. This study demonstrates omnidirectional direct ink writing (DIW) of Poly(3,4-ethylenedioxythiophene) polystyrene sulfonate (PEDOT:PSS) aerogels with tunable electrical and mechanical performance, which can be integrated with soft substrates. Several PEDOT:PSS hydrogels were formulated for DIW and freeze-dried directly on stretchable substrates to form integrated aerogels displaying high shape fidelity and minimal shrinkage. The effect of additives and processing in the PEDOT:PSS hydro and aerogels morphology, and the link with their electromechanical properties was elucidated. This technology demonstrated 3D-structured stretchable interconnects and planar thermoelectric generators (TEGs) for skin electronics, as well as vertically-printed high aspect ratio thermoelectric pillars with a high ZT value of 3.2 10^-3 and ultra-low thermal conductivity of 0.065 W/(m K). Despite their comparatively low ZT, the aerogel pillars outpowered their dense counterparts in realistic energy harvesting scenarios where contact resistances cannot be ignored, and produced up to 26 nW/cm2 (corresponding to a gravimetric power density of 0.76 mW/kg) for a difference of temperature of 15 K. This work suggests promising advancements in soft and energy-efficiency electronic systems relevant to soft robotics and wearable.",2404.12254v1 2024-05-21,Pick-and-place transfer of arbitrary-metal electrodes for van der Waals device fabrication,"Van der Waals electrode integration is a promising strategy to create near-perfect interfaces between metals and two-dimensional materials, with advantages such as eliminating Fermi-level pinning and reducing contact resistance. However, the lack of a simple, generalizable pick-and-place transfer technology has greatly hampered the wide use of this technique. We demonstrate the pick-and-place transfer of pre-fabricated electrodes from reusable polished hydrogenated diamond substrates without the use of any surface treatments or sacrificial layers. The technique enables transfer of large-scale arbitrary metal electrodes, as demonstrated by successful transfer of eight different elemental metals with work functions ranging from 4.22 to 5.65 eV. The mechanical transfer of metal electrodes from diamond onto van der Waals materials creates atomically smooth interfaces with no interstitial impurities or disorder, as observed with cross-sectional high-resolution transmission electron microscopy and energy-dispersive X-ray spectroscopy. As a demonstration of its device application, we use the diamond-transfer technique to create metal contacts to monolayer transition metal dichalcogenide semiconductors with high-work-function Pd, low-work-function Ti, and semi metal Bi to create n- and p-type field-effect transistors with low Schottky barrier heights. We also extend this technology to other applications such as ambipolar transistor and optoelectronics, paving the way for new device architectures and high-performance devices.",2405.12830v1 2013-08-15,Spin heat accumulation induced by tunneling from a ferromagnet,"An electric current from a ferromagnet into a non-magnetic material can induce a spin-dependent electron temperature. Here it is shown that this spin heat accumulation, when created by tunneling from a ferromagnet, produces a non-negligible voltage signal that is comparable to that due to the coexisting electrical spin accumulation and can give a different Hanle spin precession signature. The effect is governed by the spin polarization of the Peltier coefficient of the tunnel contact, its Seebeck coefficient, and the spin heat resistance of the non-magnetic material, which is related to the electrical spin resistance by a spin-Wiedemann-Franz law. Moreover, spin heat injection is subject to a heat conductivity mismatch that is overcome if the tunnel interface has a sufficiently large resistance.",1308.3365v2 2015-08-21,In-Plane fracture of laminated fiber reinforced composites with varying fracture resistance: experimental observations and numerical crack propagation simulations,"A series of experimental results on the in-plane fracture of a fiber reinforced laminated composite panel is analyzed using the variational multi-scale cohesive method (VMCM). The VMCM results demonstrate the influence of specimen geometry and load distribution on the propagation of large scale bridging cracks in the fiber reinforced panel. Experimentally observed variation in fracture resistance is substantiated numerically by comparing the experimental and VMCM load-displacement responses of geometrically scaled single edge-notch three point bend (SETB) specimens. The results elucidate the size dependence of the traction-separation relationship for this class of materials even in moderately large specimens, contrary to the conventional understanding of it being a material property. The existence of a ""free bridging zone"" (different from the conventional ""full bridging zone"") is recognized, and its influence on the evolving fracture resistance is discussed. The numerical simulations and ensuing bridging zone evolution analysis demonstrates the versatility of VMCM in objectively simulating progressive crack propagation, compared against conventional numerical schemes like traditional cohesive zone modeling, which require a priori knowledge of the crack path.",1508.06220v1 2016-06-17,Atomically-thin Ohmic Edge Contacts Between Two-dimensional Materials,"With the decrease of the dimensions of electronic devices, the role played by electrical contacts is ever increasing, eventually coming to dominate the overall device volume and total resistance. This is especially problematic for monolayers of semiconducting transition metal dichalcogenides (TMDs), which are promising candidates for atomically thin electronics. Ideal electrical contacts to them would require the use of similarly thin electrode materials while maintaining low contact resistances. Here we report a scalable method to fabricate ohmic graphene edge contacts to two representative monolayer TMDs - MoS2 and WS2. The graphene and TMD layer are laterally connected with wafer-scale homogeneity, no observable overlap or gap, and a low average contact resistance of 30 k$\Omega$ $\mu$m. The resulting graphene edge contacts show linear current-voltage (IV) characteristics at room temperature, with ohmic behavior maintained down to liquid helium temperatures.",1606.05393v1 2017-10-04,A phononic switch based on ferroelectric domain walls,"The ease with which domain walls (DWs) in ferroelectric materials can be written and erased provides a versatile way to dynamically modulate heat fluxes. In this work we evaluate the thermal boundary resistance (TBR) of 180$^{\circ}$ DWs in prototype ferroelectric perovskite PbTiO$_3$ within the numerical formalisms of nonequilibrium molecular dynamics and nonequilibrium Green's functions. An excellent agreement is obtained for the TBR of an isolated DW derived from both approaches, which reveals the harmonic character of the phonon-DW scattering mechanism. The thermal resistance of the ferroelectric material is shown to increase up to around 20%, in the system sizes here considered, due to the presence of a single DW, and larger resistances can be attained by incorporation of more DWs along the path of thermal flux. These results, obtained at device operation temperatures, prove the viability of an electrically actuated phononic switch based on ferroelectric DWs.",1710.01574v1 2019-09-13,Theory of anisotropic elastoresistivity of two-dimensional extremely strongly correlated metals,"There is considerable recent interest in the phenomenon of anisotropic electroresistivity of correlated metals. While some interesting work has been done on the iron-based superconducting systems, not much is known for the cuprate materials. Here we study the anisotropy of elastoresistivity for cuprates in the normal state. We present theoretical results for the effect of strain on resistivity, and additionally on the optical weight and local density of states. We use the recently developed extremely strongly correlated Fermi liquid theory in two dimensions, which accounts quantitatively for the unstrained resistivities for three families of single-layer cuprates. The strained hoppings of a tight-binding model are roughly modeled analogously to strained transition metals. The strained resistivity for a two-dimensional $t$-$t'$-$J$ model are then obtained, using the equations developed in recent work. Our quantitative predictions for these quantities have the prospect of experimental tests in the near future, for strongly correlated materials such as the hole-doped and electron-doped high-$T_c$ materials.",1909.06471v4 2020-09-04,Relation between resistance drift and optical gap in phase change materials,"The optical contrast in a phase change material is concomitant with its structural transition. We connect these two by first recognizing that Friedel oscillations couple electrons propagating in opposite directions and supply an additional Coulomb energy. As the crystal switches phase, this energy acquires time dependence and the Landau-Zener mechanism operates, steering population transfer from the valence to the conduction band and vice versa. Spectroscopy suggests that the oscillator energy dominates the optical properties and a calculation involving the crystalline field and spin-orbit interaction yields good estimates for of both structural phases. Further analysis relates the optical gap with the crystalline-field energy as well as activation energy for electrical conduction. This last property characterizes the amorphous phase, thereby furnishing a link between the crystalline field and the activation energy and ultimately with the resistance drift exponent. Providing optical means to quantify resistance drift in PCMs could circumvent the need for fabricating expensive devices and performing time consuming measurements.",2009.02048v1 2017-05-23,Reducing Graphene Device Variability with Yttrium Sacrificial Layers,"Graphene technology has made great strides since the material was isolated more than a decade ago. However, despite improvements in growth quality and numerous 'hero' devices, challenges of uniformity remain, restricting large-scale development of graphene-based technologies. Here we investigate and reduce the variability of graphene transistors by studying the effects of contact metals (with and without Ti layer), resist, and yttrium (Y) sacrificial layers during the fabrication of hundreds of devices. We find that with optical photolithography, residual resist and process contamination is unavoidable, ultimately limiting device performance and yield. However, using Y sacrificial layers to isolate the graphene from processing conditions improves the yield (from 73% to 97%), average device performance (three-fold increase of mobility, 58% lower contact resistance), and the device-to-device variability (standard deviation of Dirac voltage reduced by 20%). In contrast to other sacrificial layer techniques, removal of the Y sacrificial layer with HCl does not harm surrounding materials, simplifying large-scale graphene fabrication.",1705.09388v1 2019-10-24,Magneto-memristive switching in a two-dimensional layer antiferromagnet,"Memristive devices whose resistance can be hysteretically switched by electric field or current are intensely pursued both for fundamental interest as well as potential applications in neuromorphic computing and phase-change memory. When the underlying material exhibits additional charge or spin order, the resistive states can be directly coupled, further allowing for electrical control of the collective phases. Here, we report the observation of abrupt, memristive switching of tunneling current in nanoscale junctions of ultrathin CrI$_3$, a natural layer antiferromagnet. The coupling to spin order enables both tuning of the resistance hysteresis by magnetic field, and electric-field switching of magnetization even in multilayer samples.",1910.11383v1 2019-11-14,Nonvolatile Resistive Switching in Nanocrystalline Molybdenum Disulfide with Ion-Based Plasticity,"Non-volatile resistive switching is demonstrated in memristors with nanocrystalline molybdenum disulfide (MoS$_2$) as the active material. The vertical heterostructures consist of silicon, vertically aligned MoS$_2$ and chrome / gold metal electrodes. Electrical characterizations reveal a bipolar and forming free switching process with stable retention for at least 2500 seconds. Controlled experiments carried out in ambient and vacuum conditions suggest that the observed resistive switching is based on hydroxyl ions (OH$^-$). These originate from catalytic splitting of adsorbed water molecules by MoS$_2$. Experimental results in combination with analytical simulations further suggest that electric field driven movement of the mobile OH$^-$ ions along the vertical MoS$_2$ layers influences the energy barrier at the Si/MoS$_2$ interface. The scalable and semiconductor production compatible device fabrication process used in this work offers the opportunity to integrate such memristors into existing silicon technology for future neuromorphic applications. The observed ion-based plasticity may be exploited in ionicelectronic devices based on TMDs and other 2D materials for memristive applications.",1911.06032v1 2023-02-20,Extraordinary Bulk Insulating Behavior in the Strongly Correlated Materials FeSi and FeSb$_2$,"4$f$ electron-based topological Kondo insulators have long been researched for their potential to conduct electric current via protected surface states, while simultaneously exhibiting unusually robust insulating behavior in their interiors. To this end, we have investigated the electrical transport of the 3$d$-based correlated insulators FeSi and FeSb$_2$, which have exhibited enough similarities to their $f$ electron cousins to warrant investigation. By using a double-sided Corbino disk transport geometry, we show unambiguous evidence of surface conductance in both of these Fe-based materials. In addition, by using a 4-terminal Corbino inverted resistance technique, we extract the bulk resistivity as a function of temperature. Similar to topological Kondo insulator SmB$_6$, the bulk resistivity of FeSi and FeSb$_2$ are confirmed to exponentially increase by up to 9 orders of magnitude from room temperature to the lowest accessible temperature. This demonstrates that these materials are excellent bulk insulators, providing an ideal platform for studying correlated 2D physics.",2302.09996v1 2023-06-27,Phase transitions associated with magnetic-field induced topological orbital momenta in a non-collinear antiferromagnet,"Resistivity measurements are widely exploited to uncover electronic excitations and phase transitions in metallic solids. While single crystals are preferably studied to explore crystalline anisotropies, these usually cancel out in polycrystalline materials. Here we show that in polycrystalline Mn3Zn0.5Ge0.5N with non-collinear antiferromagnetic order, changes in the diagonal and, rather unexpected, off-diagonal components of the resistivity tensor occur at low temperatures indicating subtle transitions between magnetic phases of different symmetry. This is supported by neutron scattering and explained within a phenomenological model which suggests that the phase transitions in magnetic field are associated with field induced topological orbital momenta. The fact that we observe transitions between spin phases in a polycrystal, where effects of crystalline anisotropy are cancelled suggests that they are only controlled by exchange interactions. The observation of an off-diagonal resistivity extends the possibilities for realising antiferromagnetic spintronics with polycrystalline materials.",2306.15332v1 2023-10-20,3D Printed Architectured Silicones with Autonomic Self-healing and Creep-resistant Behavior,"Self-healing silicones that are able to restore the functionalities and extend the lifetime of soft devices hold great potential in many applications. However, currently available silicones need to be triggered to self-heal or suffer from creep-induced irreversible deformation during use. Here, we design and print silicone objects that are programmed at the molecular and architecture levels to achieve self-healing at room temperature while simultaneously resisting creep. At the molecular scale, dioxaborolanes moieties are incorporated into silicones to synthesize self-healing vitrimers, whereas conventional covalent bonds are exploited to make creep-resistant elastomers. When combined into architectured printed parts at a coarser length scale, layered materials exhibit fast healing at room temperature without compromising the elastic recovery obtained from covalent polymer networks. A patient-specific vascular phantom is printed to demonstrate the potential of architectured silicones in creating damage-resilient functional devices using molecularly designed elastomer materials.",2311.05633v1 2024-04-30,Evaluation of Thermal Performance of a Wick-free Vapor Chamber in Power Electronics Cooling,"Efficient thermal management in high-power electronics cooling can be achieved using phase-change heat transfer devices, such as vapor chambers. Traditional vapor chambers use wicks to transport condensate for efficient thermal exchange and to prevent ""dry-out"" of the evaporator. However, wicks in vapor chambers present significant design challenges arising out of large pressure drops across the wicking material, which slows down condensate transport rates and increases the chances for dry-out. Thicker wicks add to overall thermal resistance, while deterring the development of thinner devices by limiting the total thickness of the vapor chamber. Wickless vapor chambers eliminate the use of metal wicks entirely, by incorporating complementary wettability-patterned flat plates on both the evaporator and the condenser side. Such surface modifications enhance fluid transport on the evaporator side, while allowing the chambers to be virtually as thin as imaginable, thereby permitting design of thermally efficient thin electronic cooling devices. While wick-free vapor chambers have been studied and efficient design strategies have been suggested, we delve into real-life applications of wick-free vapor chambers in forced air cooling of high-power electronics. An experimental setup is developed wherein two Si-based MOSFETs of TO-247-3 packaging having high conduction resistance, are connected in parallel and switched at 100 kHz, to emulate high frequency power electronics operations. A rectangular copper wick-free vapor chamber spreads heat laterally over a surface 13 times larger than the heating area. This chamber is cooled externally by a fan that circulates air at room temperature. The present experimental setup extends our previous work on wick-free vapor chambers, while demonstrating the effectiveness of low-cost air cooling in vapor-chamber enhanced high-power electronics applications.",2404.19195v1 2017-07-26,Particle acceleration with anomalous pitch angle scattering in 2D MHD reconnection simulations,"The conversion of magnetic energy into other forms during solar flares is one of the outstanding open problems in solar physics. It is generally accepted that magnetic reconnection plays a crucial role in these conversion processes. To achieve the rapid energy release required in solar flares, an anomalous resistivity, orders of magnitude higher than the Spitzer resistivity, is often used in MHD simulations of reconnection. Spitzer resistivity is based on Coulomb scattering, which becomes negligible at the high energies achieved by accelerated particles. As a result, simulations of particle acceleration in reconnection events are often performed in the absence of any interaction between accelerated particles and any background plasma. This need not be the case for scattering associated with anomalous resistivity caused by turbulence within solar flares, as the higher resistivity implies an elevated scattering rate. We present results of test particle calculations, with and without pitch angle scattering, subject to fields derived from MHD simulations of two-dimensional (2D) X-point reconnection. Scattering rates proportional to the ratio of the anomalous resistivity to the local Spitzer resistivity, as well as at fixed values, are considered. Pitch angle scattering, which is independent of the anomalous resistivity, causes higher maximum energies in comparison to those obtained without scattering. Scattering rates which are dependent on the local anomalous resistivity tend to produce fewer highly energised particles due to weaker scattering in the separatrices, even though scattering in the current sheet may be stronger when compared to resistivity-independent scattering. Strong scattering also causes an increase in the number of particles exiting the computational box in the reconnection outflow region, as opposed to along the separatrices as is the case in the absence of scattering.",1709.00305v1 2023-02-04,"Smooth, homogeneous, high-purity Nb3Sn superconducting RF resonant cavity by seed-free electrochemical synthesis","Workbench-size particle accelerators, enabled by Nb3Sn-based superconducting radio-frequency (SRF) cavities, hold the potential of driving scientific discovery by offering a widely accessible and affordable source of high-energy electrons and X-rays. Thin-film Nb3Sn RF superconductors with high quality factors, high operation temperatures, and high-field potentials are critical for these devices. However, surface roughness, non-stoichiometry, and impurities in Nb3Sn deposited by conventional Sn-vapor diffusion prevent them from reaching their theoretical capabilities. Here we demonstrate a seed-free electrochemical synthesis that pushes the limit of chemical and physical properties in Nb3Sn. Utilization of electrochemical Sn pre-deposits reduces the roughness of converted Nb3Sn by five times compared to typical vapor-diffused Nb3Sn. Quantitative mappings using chemical and atomic probes confirm improved stoichiometry and minimized impurity concentrations in electrochemically synthesized Nb3Sn. We have successfully applied this Nb3Sn to the large-scale 1.3 GHz SRF cavity and demonstrated ultra-low BCS surface resistances at multiple operation temperatures, notably lower than vapor-diffused cavities. Our smooth, homogeneous, high-purity Nb3Sn provides the route toward high efficiency and high fields for SRF applications under helium-free cryogenic operations.",2302.02054v2 2018-03-08,Design of a nickel-base superalloy using a neural network,"A new computational tool has been developed to model, discover, and optimize new alloys that simultaneously satisfy up to eleven physical criteria. An artificial neural network is trained from pre-existing materials data that enables the prediction of individual material properties both as a function of composition and heat treatment routine, which allows it to optimize the material properties to search for the material with properties most likely to exceed a target criteria. We design a new polycrystalline nickel-base superalloy with the optimal combination of cost, density, gamma' phase content and solvus, phase stability, fatigue life, yield stress, ultimate tensile strength, stress rupture, oxidation resistance, and tensile elongation. Experimental data demonstrates that the proposed alloy fulfills the computational predictions, possessing multiple physical properties, particularly oxidation resistance and yield stress, that exceed existing commercially available alloys.",1803.03039v1 2023-04-22,Studies of two-dimensional material resistive random-access memory by kinetic Monte Carlo simulations,"Resistive memory based on 2D WS2, MoS2, and h-BN materials has been studied, including experiments and simulations. The influences with different active layer thicknesses have been discussed, including experiments and simulations. The thickness with the best On/Off ratio is also found for the 2D RRAM. This work reveals fundamental differences between a 2D RRAM and a conventional oxide RRAM. Furthermore, from the physical parameters extracted with the KMC model, the 2D materials have a lower diffusion activation energy from the vertical direction, where a smaller bias voltage and a shorter switching time can be achieved. It was also found the diffusion activation energy from the CVD-grown sample is much lower than the mechanical exfoliated sample. The result shows MoS2 has the fastest switching speed among three 2D materials.",2304.11345v2 2018-11-25,Atomic mechanisms of fast diffusion of large atoms in Germanium,"The performance of strained silicon as the channel material for transistors has plateaued. Motivated by increasing charge-carrier mobility within the device channel to improve transistor performance, germanium (Ge) is considered as an attractive option as a silicon replacement due to its highest p-type mobility in all of the known semiconductor materials and being compatible with today's conventional CMOS manufacturing process. However, the intrinsically high carrier mobility of Ge becomes significantly degraded because Ge's native oxide is unstable and readily decomposes into several GexOy suboxides with a high density of dangling bonds at the surface. In addition, these interface trap states will also degrade the off-state leakage current and subthreshold turn-off of a Ge-based device, significantly affecting its stability. Furthermore, obtaining low-resistance Ohmic contacts to n-type Ge is another key challenge in developing Ge CMOS. To solve these challenges, extensive efforts have been made about the incorporation of new materials, such as Al2O3, SiN3, TiO2, ZnO, Ge3N4, MgO, HfO2, SrTiO3, and Y2O3, into Ge transistors. Controlling the diffusion of foreign atoms into Ge is therefore a critical issue in developing Ge transistors regarding that foreign impurities may be detrimental to devices. In this work, we study the diffusion properties of all common elements in Ge by performing the first-principle calculations with a nudged elastic band method. We find some large atoms, such as Cu, Au, Pd, etc., have a very small diffusion barrier. We reveal the underlying mechanism in a combination of local distortion induced by size effect and bonding effect that controls the diffusion behaviors of different atoms in Ge. This comprehensive study and relatively in-depth understanding of diffusion in Ge provides us with a practical guide for utilizing it more efficiently in semiconductor devices.",1811.10046v1 2022-07-29,Reactive Two-Step Additive Manufacturing of Ultra-high Temperature Carbide Ceramics,"Ultra-high-temperature ceramics (UHTCs) are candidate structural materials for applications that require resiliency to extreme temperature (>2000{\deg}C), high mechanical loads, or aggressive oxidizing environments. Processing UHTC transition metal carbides as standalone materials using additive manufacturing (AM) methods has not been fully realized due to their extremely slow atomic diffusivities that impede sintering and large volume changes during indirect AM that can induce defect structures. In this work, a two-step, reactive AM approach was studied for the formation of the ultra-high temperature ceramic TiCx. Readily available equipment including a polymer powder bed fusion AM machine and a traditional tube furnace were used to produce UHTC cubes and lattice structures with sub-millimeter resolution. This processing scheme incorporated, (1) selective laser sintering of a Ti precursor mixed with a phenolic binder for green body shaping, and (2) ex-situ, isothermal gas-solid conversion of the green body in CH4 to form TiCx structures. Reactive post-processing in CH4 resulted in up to 98.2 wt% TiC0.90 product yield and a reduction in net-shrinkage during consolidation due to the volume expansion associated with the conversion of Ti to TiC. Results indicated that reaction bonding associated with the Gibbs free energy release associated with TiC formation produced interparticle adhesion at low furnace processing temperatures. The ability to bond highly refractory materials through this type of process resulted in structures that were crack-free and resisted fracture during thermal shock testing. Broadly, the additive manufacturing approach presented could be useful for the production of many UHTC carbides that might otherwise be incompatible with prevailing AM techniques that do not include reaction synthesis.",2208.00052v3 2003-05-29,Structural and electrical properties of tantalum nitride thin films fabricated by using reactive radio-frequency magnetron sputtering,"TaN thin film is an attractive interlayer as well as a diffusion barrier layer in [FeN/TaN](n) multilayers for the application as potential write-head materials in high-density magnetic recording. We synthesized two series of TaN films on glass and Si substrates by using reactive radio-frequency sputtering under 5-mtorr Ar/N-2 processing pressure with varied N-2 partial pressure, and carried out systematic characterization analyses of the films. We observed clear changes of phases in the films from metallic bcc Ta to a mixture of bcc Ta(N) and hexagonal Ta2N, then sequentially to fcc TaN and a mixture of TaN with N-rich phases when the N2 partial pressure increased from 0.0% to 30%. The changes were associated with changes in the grain shapes as well as in the preferred crystalline orientation of the films from bcc Ta [100] to [110], then to random and finally to fcc TaN [111], correspondingly. They were also associated with a change in film resistivity from metallic to semiconductor-like behavior in the range of 77-295 K. The films showed a typical polycrystalline textured structure with small, crystallized domains and irregular grain shapes. Clear preferred (111) stacks parallel to the substrate surface with embedded amorphous regions were observed in the film. TaN film with [ 111]-preferred orientation and a resistivity of 6.0 m Omega cm was obtained at 25% N-2 partial pressure, which may be suitable for the interlayer in [FeN/TaN](n) multilayers.",0305683v2 2011-12-08,"Structural, Thermal, Magnetic and Electronic Transport Properties of the LaNi2(Ge{1-x}P{x})2 System","Polycrystalline samples of LaNi2(Ge{1-x}P{x})2 (x = 0, 0.25, 0.50, 0.75, 1) were synthesized and their properties investigated by x-ray diffraction (XRD), heat capacity Cp, magnetic susceptibility chi, and electrical resistivity rho measurements versus temperature T. These compounds all crystallize in the body-centered-tetragonal ThCr2Si2-type structure. The rho(T) measurements indicate that all compositions in this system are metallic. The low-T Cp measurements yield a rather large Sommerfeld coefficient gamma = 12.4(2) mJ/mol K^2 for x = 0 reflecting a large density of states at the Fermi energy that is comparable with the largest values found for the AFe2As2 class of materials with the same crystal structure. The gamma decreases approximately linearly with x to 7.4(1) mJ/mol K^2 for x = 1. The chi measurements show nearly temperature-independent paramagnetic behavior across the entire range of compositions except for LaNi2Ge2, where a broad peak is observed at 300 K from chi(T) measurements up to 1000 K that may arise from short-range antiferromagnetic correlations in a quasi-two-dimensional magnetic system. High-accuracy Pade approximants representing the Debye lattice heat capacity and Bloch-Gruneisen electron-phonon resistivity functions versus T are presented and are used to analyze our experimental Cp(T) and rho(T) data, respectively. The T-dependences of rho for all samples are well-described by the Bloch-Gruneisen model, although the observed rho(300 K) values are larger than calculated from this model. A significant T-dependence of the Debye temperature determined from the Cp(T) data was observed for each composition. No clear evidence for bulk superconductivity or any other long-range phase transition was found for any of the compositions studied.",1112.1864v2 2013-08-14,Stable pseudoanalytical computation of electromagnetic fields from arbitrarily-oriented dipoles in cylindrically stratified media,"Computation of electromagnetic fields due to point sources (Hertzian dipoles) in cylindrically stratified media is a classical problem for which analytical expressions of the associated tensor Green's function have been long known. However, under finite-precision arithmetic, direct numerical computations based on the application of such analytical (canonical) expressions invariably lead to underflow and overflow problems related to the poor scaling of the eigenfunctions (cylindrical Bessel and Hankel functions) for extreme arguments and/or high-order, as well as convergence problems related to the numerical integration over the spectral wavenumber and to the truncation of the infinite series over the azimuth mode number. These problems are exacerbated when a disparate range of values is to be considered for the layers' thicknesses and material properties (resistivities, permittivities, and permeabilities), the transverse and longitudinal distances between source and observation points, as well as the source frequency. To overcome these challenges in a systematic fashion, we introduce herein different sets of range-conditioned, modified cylindrical functions (in lieu of standard cylindrical eigenfunctions), each associated with non-overlapped subdomains of (numerical) evaluation to allow for stable computations under any range of physical parameters. In addition adaptively-chosen integration contours are employed in the complex spectral wavenumber plane to ensure convergent numerical integration in all cases. We illustrate the application of the algorithm to problems of geophysical interest involving layer resistivities ranging from 1000 $\Omega \cdot$m to 10$^{-8} \Omega \cdot$m, frequencies of operation ranging from 10 MHz down to the low magnetotelluric range of 0.01 Hz, and for various combinations of layer thicknesses.",1308.3179v2 2019-03-01,Coexistence of metallic and nonmetallic properties in the pyrochlore Lu$_2$Rh$_2$O$_7$,"Transition metal oxides of the $4d$ and $5d$ block have recently become the targets of materials discovery, largely due to their strong spin-orbit coupling that can generate exotic magnetic and electronic states. Here we report the high pressure synthesis of Lu$_2$Rh$_2$O$_7$, a new cubic pyrochlore oxide based on $4d^5$ Rh$^{4+}$ and characterizations via thermodynamic, electrical transport, and muon spin relaxation measurements. Magnetic susceptibility measurements reveal a large temperature-independent Pauli paramagnetic contribution, while heat capacity shows an enhanced Sommerfeld coefficient, $\gamma$ = 21.8(1) mJ/mol-Rh K$^2$. Muon spin relaxation measurements confirm that Lu$_2$Rh$_2$O$_7$ remains paramagnetic down to 2 K. Taken in combination, these three measurements suggest that Lu$_2$Rh$_2$O$_7$ is a correlated paramagnetic metal with a Wilson ratio of $R_W = 2.5$. However, electric transport measurements present a striking contradiction as the resistivity of Lu$_2$Rh$_2$O$_7$ is observed to monotonically increase with decreasing temperature, indicative of a nonmetallic state. Furthermore, although the magnitude of the resistivity is that of a semiconductor, the temperature dependence does not obey any conventional form. Thus, we propose that Lu$_2$Rh$_2$O$_7$ may belong to the same novel class of non-Fermi liquids as the nonmetallic metal FeCrAs.",1903.00399v1 2022-01-10,"Alloyed B-(AlxGa1-x)2O3 bulk Czochralski single B-(Al0.1Ga0.9)2O3 and polycrystals B-(Al0.33Ga0.66)2O3, B-(Al0.5Ga0.5)2O3), and property trends","In this work, bulk Czochralski-grown single crystals of 10 mol. % Al2O3 alloyed B-Ga2O3 - monoclinic 10% AGO or B-(Al0.1Ga0.9)2O3 - are obtained, which show +0.20 eV increase in the bandgap compared with unintentionally doped B-Ga2O3. Further, growths of 33% AGO - B-(Al0.33Ga0.67)2O3 - and 50% AGO - B-(Al0.5Ga0.5)2O3 or B-AlGaO3 - produce polycrystalline single-phase monoclinic material (B-AGO). All three compositions are investigated by x-ray diffraction, Raman spectroscopy, optical absorption, and 27Al nuclear magnetic resonance (NMR). By investigating single phase B-AGO over a large range of Al2O3 concentrations (10 - 50 mol. %), broad trends in the lattice parameter, vibrational modes, optical bandgap, and crystallographic site preference are determined. All lattice parameters show a linear trend with Al incorporation. According to NMR, aluminum incorporates on both crystallographic sites of B-Ga2O3, with a slight preference for the octahedral (GaII) site, which becomes more disordered with increasing Al. Single crystals of 10% AGO were also characterized by x-ray rocking curve, transmission electron microscopy, purity (glow discharge mass spectroscopy and x-ray fluorescence), optical transmission (200 nm - 20 um wavelengths), and resistivity. These measurements suggest that electrical compensation by impurity acceptor doping is not the likely explanation for high resistivity, but rather the shift of a hydrogen level from a shallow donor to a deep acceptor due to Al alloying. .. Cont. This article may be downloaded for personal use only. Any other use requires prior permission of the author and AIP Publishing. This article appeared in Journal of Applied Physics 131 155702.",2201.03673v2 2023-02-09,Spark Discharge Generator as a Stable and Reliable Nanoparticle Synthesis Device: Analysis of the Impact of Process and Circuit Variables on the Characteristics of Synthesized Nanoparticles,"Nanotechnology offers the promise of harnessing quantum properties not available in the bulk phase. These desirable properties are highly dependent on size and composition. Generators that control these variables are therefore essential for progress in the field. The spark discharge generator (SDG) is an outstanding aerosol route for nanoparticle synthesis, which stands out due to its fast kinetics, scalability, high purity, accuracy and reproducibility with the added advantage of allowing the synthesis of nanoparticles of any conducting material. These advantages are a consequence of its vast heating and cooling rates, its intrinsic and easily controllable electronic variables at the reach of a click. However, the mechanistic impact of these variables on the actual aerosol generated is still not fully understood. In this work, we constructed an SDG and systematically studied its behavior with particular interest in the effect that resistance, capacitance, inductance, flow rate, gap separation and current have on the electrical behavior of the spark. Our model system produced primarily Fe and Cu nanoparticles with measured concentrations. We discuss how the spark influences particle size and number concentration and provide useful correlations that link dependent with independent variables. Remarkably, a finite resistance produces a maximum in the output of the generated aerosols. This suggests a direct link between RLC properties of the circuit and cabling into the frequency of the spark, and nanoparticle number concentration, indicating potential for exploiting such behavior towards maximizing nanoparticle generation. Furthermore, we discuss a link between spark oscillations and energy release with its consequent aerosol generation.",2302.04760v1 2013-08-08,"Ultra-low Energy, High-Performance Dynamic Resistive Threshold Logic","We propose dynamic resistive threshold-logic (DRTL) design based on non-volatile resistive memory. A threshold logic gate (TLG) performs summation of multiple inputs multiplied by a fixed set of weights and compares the sum with a threshold. DRTL employs resistive memory elements to implement the weights and the thresholds, while a compact dynamic CMOS latch is used for the comparison operation. The resulting DRTL gate acts as a low-power, configurable dynamic logic unit and can be used to build fully pipelined, high-performance programmable computing blocks. Multiple stages in such a DRTL design can be connected using energy-efficient low swing programmable interconnect networks based on resistive switches. Owing to memory-based compact logic and interconnect design and highspeed dynamic-pipelined operation, DRTL can achieve more than two orders of magnitude improvement in energy-delay product as compared to look-up table based CMOS FPGA.",1308.4672v1 2013-10-11,Curvature dependence of the interfacial heat and mass transfer coefficients,"Nucleation is often accompanied by heat transfer between the surroundings and a nucleus of a new phase. The interface between two phases gives an additional resistance to this transfer. For small nuclei the interfacial curvature is high, which affects not only equilibrium quantities such as surface tension, but also the transport properties. In particular, high curvature affects the interfacial resistance to heat and mass transfer. We develop a framework for determining the curvature dependence of the interfacial heat and mass transfer resistances. We determine the interfacial resistances as a function of a curvature. The analysis is performed for a bubble of a one-component fluid and may be extended to various nuclei of multicomponent systems. The curvature dependence of the interfacial resistances is important in modeling transport processes in multiphase systems.",1310.3025v1 2014-08-30,Anisotropic resistivity of the monolayer graphene in the trigonal warping and connected Fermi curve regimes,"In the present study, the anisotropic resistivity of the monolayer graphene has been obtained in semiclassical regime beyond the Dirac point approximation. In particular, detailed investigations were made on the dependence of conductivity on the Fermi energy. At low energies, in the vicinity of the Dirac points, band energy of the monolayer graphene is isotropic at the Fermi level. Meanwhile, at the intermediate Fermi energies anisotropic effects such as trigonal warping is expected to be the origin of the anisotropic resistivity. However, besides the band anisotropy there also exists an other source of anisotropic resistivity which was introduced by scattering matrix. At high energies it was shown that the band anisotropy is less effective than the anisotropy generated by the scattering matrix. It was also shown that there exist two distinct regimes of anisotropic resistivity corresponding the trigonal warping and connected Fermi curve at intermediate and high energies respectively.",1409.0130v1 2018-08-19,Temperature Dependence of In-plane Resistivity and Inverse Hall Angle in NLED Holographic Model,"In the strange metal phase of the high-$T_{c}$ cuprates, it is challenging to explain the linear temperature dependence of the in-plane resistivity and the quadratic temperature dependence of the inverse Hall angle. In this paper, we investigate the temperature dependence of the in-plane resistivity and inverse Hall angle in the nonlinear electrodynamics holographic model developed in our recent work. Maxwell electrodynamics and Born-Infeld electrodynamics are considered. Both cases support a wide spectrum of temperature scalings in parameter space. For Maxwell electrodynamics, the T-linear in-plane resistivity generally dominates at low temperatures and survives into higher temperatures in a narrow strip-like manner. Meanwhile, the T-quadratic inverse Hall angle dominates at high temperatures and extends down to lower temperatures. The overlap between the T-linear in-plane resistivity and the T-quadratic inverse Hall angle, if occurs, would generally present in the intermediate temperate regime. The Born-Infeld case with $a>0$ is quite similar to the Maxwell case. For the Born-Infeld case with $a<0$, there can be a constraint on the charge density and magnetic field. Moreover, the overlap can occur for strong charge density.",1808.06158v1 2019-04-18,Non-Stationary Polar Codes for Resistive Memories,"Resistive memories are considered a promising memory technology enabling high storage densities with in-memory computing capabilities. However, the readout reliability of resistive memories is impaired due to the inevitable existence of wire resistance, resulting in the sneak path problem. Motivated by this problem, we study polar coding over channels with different reliability levels, termed non-stationary polar codes, and we propose a technique improving its bit error rate (BER) performance. We then apply the framework of non-stationary polar codes to the crossbar array and evaluate its BER performance under two modeling approaches, namely binary symmetric channels (BSCs) and binary asymmetric channels (BSCs). Finally, we propose a technique for biasing the proportion of high-resistance states in the crossbar array and show its advantage in reducing further the BER. Several simulations are carried out using a SPICE-like simulator, exhibiting significant reduction in BER.",1904.08966v1 2019-12-06,Write and Read Channel Models for 1S1R Crossbar Resistive Memory with High Line Resistance,"Crossbar resistive memory with 1 Selector 1 Resistor (1S1R) structure is attractive for low-cost and high-density nonvolatile memory applications. As technology scales down to the single-nm regime, the increasing resistivity of wordline/bitline becomes a limiting factor to device reliability. This paper presents write/read communication channels while considering the line resistance and device variabilities by statistically relating the degraded write/read margins and the channel parameters. Binary asymmetric channel (BAC) models are proposed for the write/read operations. Simulations based on these models suggest that the bit-error rate of devices are highly non-uniform across the memory array. These models provide quantitative tools for evaluating the trade-offs between memory reliability and design parameters, such as array size, technology nodes, and aspect ratio, and also for designing coding-theoretic solutions that would be most effective for crossbar memory.",1912.02963v3 2020-05-15,Anomalous Electrical Conduction and Negative Temperature Coefficient of Resistance in Nanostructured Gold Resistive Switching Films,"We report on the observation of non-metallic electrical conduction, resistive switching, and a negative temperature coefficient of resistance in cluster-assembled nanostructured gold films above the electrical percolation and in strong-coupling regime, from room to cryogenic temperatures (24K). The structure of the films is characterized by an extremely high density of randomly oriented crystalline nanodomains, separated by grain boundaries. The observed behavior can be explained by considering space charge limited conduction and Coulomb blockade phenomena highlighting the influence of the high density of defects and grain boundaries on the localization of conduction electrons. Our findings have implications for a broad class of resistive switching systems based on random assemblies of nanoobjects.",2005.07401v1 2021-05-22,Dynamic-quenching of a single-photon avalanche photodetector using an adaptive resistive switch,"One of the most common approaches for quenching single-photon avalanche diodes is to use a passive resistor in series with it. A drawback of this approach has been the limited recovery speed of the single-photon avalanche diodes. High resistance is needed to quench the avalanche, leading to slower recharging of the single-photon avalanche diodes depletion capacitor. We address this issue by replacing a fixed quenching resistor with a bias-dependent adaptive resistive switch. Reversible generation of metallic conduction enables switching between low and high resistance states under unipolar bias. As an example, using a Pt/Al2O3/Ag resistor with a commercial silicon single-photon avalanche diodes, we demonstrate avalanche pulse widths as small as ~30 ns, 10x smaller than a passively quenched approach, thus significantly improving the single-photon avalanche diodes frequency response. The experimental results are consistent with a model where the adaptive resistor dynamically changes its resistance during discharging and recharging the single-photon avalanche diodes.",2105.11454v2 2022-09-14,Picosecond Time-Scale Resistive Switching Monitored in Real-Time,"The resistance state of filamentary memristors can be tuned by relocating only a few atoms at interatomic distances in the active region of a conducting filament. Thereby the technology holds promise not only in its ultimate downscaling potential and energy efficiency but also in unprecedented speed. Yet, the breakthrough in high-frequency applications still requires the clarification of the dominant mechanisms and inherent limitations of ultra-fast resistive switching. Here we investigate bipolar, multilevel resistive switchings in tantalum pentoxide based memristors with picosecond time resolution. We experimentally demonstrate cyclic resistive switching operation due to 20 ps long voltage pulses of alternating polarity. Through the analysis of the real-time response of the memristor we find that the set switching can take place at the picosecond time-scale where it is only compromised by the bandwidth limitations of the experimental setup. In contrast, the completion of the reset transitions significantly exceeds the duration of the ultra-short voltage bias, demonstrating the dominant role of thermal diffusion and underlining the importance of dedicated thermal engineering for future high-frequency memristor circuit applications.",2209.06732v1 2022-12-02,Nondestructive KPFM-assisted Quality Control in Fabrication of GaAs High-Speed Electronics,"In this paper, we report on the method of nondestructive quality control that can be used in fabrication of GaAs high-speed electronics. The method relies on the surface potential mapping and enables rigid in vivo analysis of transport properties of an active electronic device incorporated into a complex integrated circuit. The study is inspired by our ongoing development of a millimeter wave intelligent reflective surface for 6G communications. To provide desired beamforming capabilities, such a surface should utilize hundreds of identical microscale GaAs diode switches with series resistance of a few ohms. Thus, we develop a ladder-like layered ohmic contact to heavily Si-doped GaAs and cross-study it via transmission line method and Kelvin probe force microscopy. The contact resistivity as low as 0.15~$\mu \Omega \,$cm$^2$ is measured resulting in only a 0.6~$\Omega$ of resistance for the contact area of 3$\times$3~$\mu$m$^2$. Moreover, the tendencies observed suggest that one can rigidly analyze the evolution of contact resistance and the profile of resistivity under contact in response to rapid thermal annealing, once the surface potential map across the ``ladder'' is known.",2212.01474v1 2023-09-22,Terahertz scale microbunching instability driven by nonevaporable getter coating resistive-wall impedance,"Non-evaporable getter (NEG) coating is widely required in the next generation of light sources and circular $e^+e^-$ colliders for small vacuum pipes to improve the vacuum level, which, however, also enhances the high-frequency resistive-wall impedance and often generates a resonator-like peak in the terahertz frequency region. In this paper, we will use the parameters of the planned Hefei Advanced Light Facility (HALF) storage ring to study the impact of NEG coating resistive-wall impedance on the longitudinal microwave instability via particle tracking simulation. Using different NEG coating parameters (resistivity and thickness) as examples, we find that the impedance with a narrow and strong peak in the high frequency region can cause micro-bunching instability, which has a low instability threshold current and contributes to a large energy spread widening above the threshold. In order to obtain a convergent simulation of the beam dynamics, one must properly resolve such a peak. The coating with a lower resistivity has a much less sharp peak in its impedance spectrum, which is helpful to suppress the micro-bunching instability and in return contributes to a weaker microwave instability.",2309.12779v1 2024-04-29,Evolution of secondary electron spectrum during cosmic-ray discharge in the universe,"We recently found that streaming cosmic rays (CRs) induce a resistive electric field that can accelerate secondary electrons produced by CR ionization. In this work, we study the evolution of the energy spectrum of secondary electrons by numerically solving the one-dimensional Boltzmann equation and Ohm's law. We show that the accelerated secondary electrons further ionize a gas, that is, the electron avalanche occurs, resulting in increased ionization and excitation of the gas. Although the resistive electric field becomes weaker than one before the CR discharge, the weak resistive electric field weakly accelerates the secondary electrons. The quasi-steady state is almost independent of the initial resistive electric field, but depends on the electron fraction in the gas. The resistive electric field in the quasi-steady state is larger for the higher electron fraction, which makes the number of secondary electrons that can ionize the gas larger, resulting in a higher ionization rate. The CR discharge could explain the high ionization rate that are observed in some molecular clouds.",2404.18513v1 2007-03-26,An alternative normal state c-axis resistivity model for high-Tc superconductors,"An alternative model for c-axis resistivity in layered high-Tc crystalline superconductors is proposed and has been characterized as an essentially two-dimensional Fermi liquid. Average ionization energy is included as additional parameter that determines the concentration of tunnelling electrons between Cu-O2 layers. This model agrees well quantitatively with the Bi2212 and Y123 single crystals, and qualitatively with the pure 1212 phase polycrystals.",0703658v1 2005-02-02,Phase transitions in Lu$_2$Ir$_3$Si$_5$,"We report the results of our investigations on a polycrystalline sample of Lu$_2$Ir$_3$Si$_5$ which crystallizes in the U$_2$Co$_3$Si$_5$ type structure (Ibam). These investigations comprise powder X-ray diffraction, magnetic susceptibility, electrical resistivity and high temperature (120-300 K) heat capacity studies. Our results reveal that the sample undergoes a superconducting transition below 3.5 K. It also undergoes a first order phase transition between 150-250 K as revealed by an upturn in the resistivity, a diasmagnetic drop in the magnetic susceptibility and a large anomaly (20-30 J/mol K) in the specific heat data. We observe a huge thermal hysteresis of almost 45 K between the cooling and warming data across this high temperature transition in all our measurements. Low temperature X-ray diffraction measurements at 87 K reveals that the compound undergoes a structural change at the high temperature transition. Resistivity data taken in repeated cooling and warming cycles indicate that at the high temperature transition, the system goes into a highly metastable state and successive heating/cooling curves are found to lie above the previous one and the resistance keeps increasing with every thermal cycle. The room temperature resistance of a thermaly cycled piece of the sample decays exponentialy with time with a decay time constant estimated to be about 10$^4$ secs. The anomaly (upturn) in the resistivity and the large drop (almost 45%) in the susceptibility across the high temperature transition suggest that the observed structural change is accompanied or induced by an electronic transition.",0502041v2 2014-06-23,Resistance of helical edges formed in a semiconductor heterostructure,"Time-reversal symmetry prohibits elastic backscattering of electrons propagating within a helical edge of a two-dimensional topological insulator. However, small band gaps in these systems make them sensitive to doping disorder, which may lead to the formation of electron and hole puddles. Such a puddle -- a quantum dot -- tunnel-coupled to the edge may significantly enhance the inelastic backscattering rate, due to the long dwelling time of an electron in the dot. The added resistance is especially strong for dots carrying an odd number of electrons, due to the Kondo effect. For the same reason, the temperature dependence of the added resistance becomes rather weak. We present a detailed theory of the quantum dot effect on the helical edge resistance. It allows us to make specific predictions for possible future experiments with artificially prepared dots in topological insulators. It also provides a qualitative explanation of the resistance fluctuations observed in short HgTe quantum wells. In addition to the single-dot theory, we develop a statistical description of the helical edge resistivity introduced by random charge puddles in a long heterostructure carrying helical edge states. The presence of charge puddles in long samples may explain the observed coexistence of a high sample resistance with the propagation of electrons along the sample edges.",1406.6052v2 2016-08-03,Non-Fermi liquid behavior of electrical resistivity close to the nematic critical point in Fe$_{1-x}$Co$_x$Se and FeSe$_{1-y}$S$_y$,"Temperature dependence of resistivity of single crystals of Fe$_{1-x}$Co$_x$Se and FeSe$_{1-y}$S$_y$ is studied in detail under zero and high magnetic field (magnetoresistance), the latter of which enables to monitor the temperature ($T$) evolution of resistivity below the onset of superconducting transition temperature ($T_{\rm c}$). In FeSe$_{1-y}$S$_y$, $T$-linear dependence of resistivity is prominent in $y$ = 0.160 below 40 K, whereas it changes to a Fermi-liquid(FL)-like $T^2$ one below 10 K in $y$ = 0.212. These suggest that the quantum critical point (QCP) originating from the electronic nematicity resides around $y$ = 0.160 and the fluctuation in QCP gives rise anomalous $T$-linear dependence in resistivity in a wide $T$ range. In Fe$_{1-x}$Co$_x$Se, resistivity gradually changes from linear- to quadratic- $T$-dependent one at low temperatures in the range between $x$ = 0.036 and 0.075. These could be interpreted by scenarios of both the nematic QCP and the crossover in the ground states between the orthorhombic nematic phase and the tetragonal phase. The anomalies found as $T$-linear resistivity are discussed in terms of orbital and spin fluctuation arising from the nematic QCP.",1608.01044v1 2017-08-01,Heterogeneous Memristive Devices Enabled by Magnetic Tunnel Junction Nanopillars Surrounded by Resistive Silicon Switches,"Emerging non-volatile memories (NVMs) have currently attracted great interest for their potential applications in advanced low-power information storage and processing technologies. Conventional NVMs, such as magnetic random access memory (MRAM) and resistive random access memory (RRAM) suffer from limitations of low tunnel magnetoresistance (TMR), low access speed or finite endurance. NVMs with synergetic advantages are still highly desired for future computer architectures. Here, we report a heterogeneous memristive device composed of a magnetic tunnel junction (MTJ) nanopillar surrounded by resistive silicon switches, named resistively enhanced MTJ (Re-MTJ), that may be utilized for novel memristive memories, enabling new functionalities that are inaccessible for conventional NVMs. The Re-MTJ device features a high ON/OFF ratio of >1000% and multilevel resistance behaviour by combining magnetic switching together with resistive switching mechanisms. The magnetic switching originates from the MTJ, while the resistive switching is induced by a point-switching filament process that is related to the mobile oxygen ions. Microscopic evidence of silicon aggregated as nanocrystals along the edges of the nanopillars verifies the synergetic mechanism of the heterogeneous memristive device. This device may provide new possibilities for advanced memristive memory and computing architectures, e.g., in-memory computing and neuromorphics.",1708.00372v2 2021-11-11,Imaging Hydrodynamic Electrons Flowing Without Landauer-Sharvin Resistance,"Electrical resistance usually originates from lattice imperfections. However, even a perfect lattice has a fundamental resistance limit, given by the Landauer conductance caused by a finite number of propagating electron modes. This resistance, shown by Sharvin to appear at the contacts of electronic devices, sets the ultimate conductance limit of non-interacting electrons. Recent years have seen growing evidence of hydrodynamic electronic phenomena, prompting recent theories to ask whether an electronic fluid can radically break the fundamental Landauer-Sharvin limit. Here, we use single-electron transistor imaging of electronic flow in high-mobility graphene Corbino disk devices to answer this question. First, by imaging ballistic flows at liquid-helium temperatures, we observe a Landauer-Sharvin resistance that does not appear at the contacts but is instead distributed throughout the bulk. This underpins the phase-space origin of this resistance - as emerging from spatial gradients in the number of conduction modes. At elevated temperatures, by identifying and accounting for electron-phonon scattering, we reveal the details of the purely hydrodynamic flow. Strikingly, we find that electron hydrodynamics eliminates the bulk Landuer-Sharvin resistance. Finally, by imaging spiraling magneto-hydrodynamic Corbino flows, we reveal the key emergent length scale predicted by hydrodynamic theories - the Gurzhi length. These observations demonstrate that electronic fluids can dramatically transcend the fundamental limitations of ballistic electrons, with important implications for fundamental science and future technologies",2111.06412v1 2022-07-30,Superconductor relaxation -- A must to be integrated into stability calculations,"A superconductor is stable if it does not quench. Quench is a short-time physics problem. For its deeper understanding of, and how to avoid quench, the physics behind stability has to be analysed. A previously suggested dynamic relaxation model is re-considered and applied to YBaCuO 123 and BSCCO 2223 high-temperature, thin film superconductors. Parallel to this investigation, an unconventional approach using an electrical resistance network (a cell model) is applied to introduce a method how to estimate the extent by which, in resistance measurements, exact determination of critical temperature of superconductors is possible. This resistive cell model, when considering its numerical convergence behaviour, in a side result may provide an alternative explanation of (at least a contribution to) bending of resistivity vs. temperature curves, and perhaps also an alternative to standard explanations of the thermal fluctuations impact on these curves. The dynamic relaxation and the resistance models provide a parenthesis that correlates, in terms of the Ginzburg-Landau order parameter, (i) solution of superconductor stability problem (the main objective of this paper), with tentative explanation of (ii) bending of the resistivity curves near critical temperature and (iii) with predictions from thermal fluctuations.",2208.00190v4 2023-09-25,Non-Volatile Resistive Switching of Polymer Residues in 2D Material Memristors,"Two-dimensional (2D) materials are popular candidates for emerging nanoscale devices, including memristors. Resistive switching (RS) in such 2D material memristors has been attributed to the formation and dissolution of conductive filaments created by the diffusion of metal ions between the electrodes. However, the area-scalable fabrication of patterned devices involves polymers that are difficult to remove from the 2D material interfaces without damage. Remaining polymer residues are often overlooked when interpreting the RS characteristics of 2D material memristors. Here, we demonstrate that the parasitic residues themselves can be the origin of RS. We emphasize the necessity to fabricate appropriate reference structures and employ atomic-scale material characterization techniques to properly evaluate the potential of 2D materials as the switching layer in vertical memristors. Our polymer-residue-based memristors exhibit RS typical for a filamentary mechanism with metal ion migration, and their performance parameters are strikingly similar to commonly reported 2D material memristors. This reveals that the exclusive consideration of electrical data without a thorough verification of material interfaces can easily lead to misinterpretations about the potential of 2D materials for memristor applications.",2309.13900v1 2023-11-14,Observation of high-temperature superconductivity in the high-pressure tetragonal phase of La2PrNi2O7-δ,"The recent discovery of high-temperature superconductivity in the Ruddlesden-Popper phase La3Ni2O7 under high pressure marks a significant breakthrough in the field of 3d transition-metal oxide superconductors. For an emerging novel class of high-Tc superconductors, it is crucial to find more analogous superconducting materials with a dedicated effort toward broadening the scope of nickelate superconductors. Here, we report on the observation of high-Tc superconductivity in the high-pressure tetragonal I4/mmm phase of La2PrNi2O7 above ~10 GPa, which is distinct from the reported orthorhombic Fmmm phase of La3Ni2O7 above 14 GPa. For La2PrNi2O7, the onset and the zero-resistance temperatures of superconductivity reach Tconset = 78.2 K and Tczero = 40 K at 15 GPa. This superconducting phase shares the samilar structural symmetry as many cuprate superconductors, providing a fresh platform to investigate underlying mechanisms of nickelate superconductors.",2311.08212v2 1999-01-11,SQUID based resistance bridge for shot noise measurement on low impedance samples,"We present a resistance bridge which uses a SQUID to measure the shot noise in low impedance samples. The experimental requirements are high DC bias currents (typically 10mA) together with high AC sensitivity (pA/VHz). This system is used to investigate the shot noise in Superconductor/Normal/Superconductor junctions where Andreev reflection enhanced shot noise is expected. Because our setup has an intrinsic noise much smaller than the thermal noise of the resistance bridge at 4.2K, reliable results can be obtained on impedances out of the range of classical measurement schemes.",9901090v2 1999-05-12,Nonmonotonic Temperature-dependent Resistance in Low Density 2D Hole Gases,"The low temperature longitudinal resistance-per-square Rxx(T) in ungated GaAs/AlGaAs quantum wells of high peak hole mobility 1.7x10^6 cm^2/Vs is metallic for 2D hole density p as low as 3.8x10^9 cm-2. The electronic contribution to the resistance, R_{el}(T), is a nonmonotonic function of T, exhibiting thermal activation, R_{el}(T) ~ exp{-E_a/kT}, for kT<EF. The form of R_{el}(T) is independent of density, indicating a fundamental relationship between the low and high T scattering mechanisms in the metallic state.",9905176v1 2005-07-28,Phononless thermally activated transport through a disordered array of quantum wires,"Phononless plasmon assisted transport through a long disordered array of finite length quantum wires is investigated analytically. Two temperature regimes, the low- and the high-temperature ones, with qualitatively different temperature dependencies of thermally activated resistance are identified. The characteristics of plasmon assisted and phonon assisted transport mechanisms are compared. Generically strong electron-electron interaction in quantum wires results in a qualitative change of the temperature dependence of thermally activated resistance in comparison to phonon assisted transport. At high temperatures, the thermally activated resistance is determined by the Luttinger liquid interaction parameter of the wires.",0507687v1 2007-02-22,High-field Hall resistivity and magnetoresistance in electron-doped Pr_2-xCe_xCuO_{4-δ},"We report resistivity and Hall effect measurements in electron-doped Pr$_{2-x}$Ce$_{x}$CuO$_{4-\delta}$ films in magnetic field up to 58 T. In contrast to hole-doped cuprates, we find a surprising non-linear magnetic field dependence of Hall resistivity at high field in the optimally doped and overdoped films. We also observe a crossover from quadratic to linear field dependence of the positive magnetoresistance in the overdoped films. A spin density wave induced Fermi surface reconstruction model can be used to qualitatively explain both the Hall effect and magnetoresistance.",0702534v2 2007-01-13,First Tests of Thick GEMs with Electrodes Made of a Resistive Kapton,"We have developed a new design of a GEM-like detector with single-layer electrodes made of a resistive kapton. This detector can operate at gains close to 10E5 even in pure Ar and Ne and if transited to discharges at higher gains they, due to the high resistivity of electrodes, do not damage either the detector or the front-end electronics. Gains ~ 106 can be achieved in a cascaded mode of the operation. The detector can operate without gain degradation at counting rates up to 10E4Hz/cm2 and thus it could be very useful in many applications which require safe high gain operation, for example in RICH, TPCs, calorimetric.",0701154v1 1995-07-03,Percolation transition of the vortex lattice and c-axis resistivity in high-temperature superconductors,"We use the three-dimensional Josephson junction array system as a model for studying the temperature dependence of the c-axis resistivity of high temperature superconductors, in the presence of an external magnetic field H applied in the c-direction. We show that the temperature at which the dissipation becomes different from zero corresponds to a percolation transition of the vortex lattice. In addition, the qualitative features of the resistivity vs. temperature curves close to the transition are obtained starting from the geometrical configurations of the vortices. The results apply to the cases H greater than 0 and H=0.",9507001v1 2007-06-21,"Addendum: ""On the nature of the phase transition in the itinerant helimagnet MnSi"", arXiv:cond-mat/0702460v1 [cond-mat.str-el]","New high resolution data for heat capacity, heat capacity under applied magnetic fields and resistivity of high quality single crystal of MnSi are reported. Striking mirror symmetry between temperature derivative of resistivity and thermal expansion coefficient of MnSi is displayed. Close similarity between variation of the heat capacity and the temperature derivative of resistivity through the phase transition is observed. It is shown that the heat capacity and thermal expansion coefficient of the helical phase are not influenced by moderate magnetic field.",0706.3093v1 2009-02-24,Phonon-induced Resistance Oscillations in Very-high Mobility 2D Electron Systems,"We report on temperature dependence of acoustic phonon-induced resistance oscillations in very high mobility two-dimensional electron systems. We observe that the temperature dependence is non-monotonic and that higher order oscillations are best developed at progressively lower temperatures. Our analysis shows that, in contrast to Shubnikov-de Haas effect, phonon-induced resistance oscillations are sensitive to electron-electron interactions modifying the single particle lifetime.",0902.4208v1 2009-09-11,Resistive g-modes in a reversed field pinch plasma,"First direct experimental evidence of high frequency, high toroidal mode number (n>20), magnetic fluctuations due to unstable resistive interchange modes (g-modes) resonant in the edge region of a reversed field pinch (RFP) plasma is presented. Experimental characterization of time and space periodicities of the modes is provided by means of highly resolved in-vessel edge and insertable magnetic diagnostics. It is found that the spectral mode properties are in good agreement with the predictions of the theoretical linear resistive magnetohydrodynamic stability analysis. A simple model is proposed for the observed saturation levels of the modes.",0909.2153v1 2010-07-16,Zero differential resistance in two-dimensional electron systems at large filling factors,"We report on a state characterized by a zero differential resistance observed in very high Landau levels of a high-mobility two-dimensional electron system. Emerging from a minimum of Hall field-induced resistance oscillations at low temperatures, this state exists over a continuous range of magnetic fields extending well below the onset of the Shubnikov-de Haas effect. The minimum current required to support this state is largely independent on the magnetic field, while the maximum current increases with the magnetic field tracing the onset of inter-Landau level scattering.",1007.2832v1 2013-10-09,Effect of Temperature and Charged Particle Fluence on the Resistivity of Polycrystalline CVD Diamond Sensors,"The resistivity of polycrystalline chemical vapor deposition diamond sensors is studied in samples exposed to fluences relevant to the environment of the High Luminosity Large Hadron Collider. We measure the leakage current for a range of bias voltages on samples irradiated with 800 MeV protons up to 1.6\times 10^{16} p/cm^2. The proton beam at LANSCE, Los Alamos National Laboratory, was applied to irradiate the samples. The devices' resistivity is extracted for temperatures in the -10^\circC to +20^\circC range.",1310.2620v1 2016-07-04,Vortex motion and flux-flow resistivity in dirty multiband superconductors,"The conductivity of vortex lattices in multiband superconductors with high concentration of impurities is calculated based on microscopic kinetic theory. Both the limits of high and low fields are considered, when the magnetic induction is close to or much smaller than the critical field strength $H_{c2}$, respectively. It is shown that in contrast to single-band superconductors the resistive properties are not universal but depend on the pairing constants and ratios of diffusivities in different bands. The low-field magneto-resistance can strongly exceed Bardeen-Stephen estimation in a quantitative agreement with experimental data for two-band superconductor MgB$_2$.",1607.00708v2 2023-02-27,Ferromagnetism and Metal-Insulator transition in F-doped LaMnO3,"We present our studies on polycrystalline samples of fluorine doped LaMnO3 (LaMnO3-yFy). LaMnO2.5F0.5 exhibits remarkable magnetic and electrical properties. It shows ferromagnetic and metallic behavior with a high Curie temperature of ~ 239 K and a high magnetoresistance of -64. This drastic change in magnetic properties in comparison to pure LaMnO3 is ascribed to the presence of mixed-valence Mn ions driven by the F-doping at the O-sites, which enables double exchange (DE) in LMOF. Furthermore, the resistivity data exhibits two resistivity peaks at 239 K and 213 K, respectively. Our results point towards the possibility of multiple double exchange hopping paths of two distinct resistances existing simultaneously in the sample below 213 K.",2302.13845v1 2009-07-25,Superconductivity in Undoped Single Crystals of BaFe2As2: Field and Current Dependence,"In previous work in undoped MFe2As2, partial drops in the resistivity indicative of traces of superconductivity have been observed in some samples of M=Ba (Tc ~ 20 K, up to 25% drop in resistivity) and M=Ca (Tc ~ 10 K, up to 45 % drop in resistivity.) A complete drop in the resistivity to 0, along with a finite fraction of Meissner flux expulsion, has been observed in M=Sr, Tc = 22 K. Using In-flux grown single crystal samples of undoped BaFe2As2, we find a complete drop in the resistivity to 0 in most samples beginning at Tc(onset) = 22.5 K. However, in contrast to the SrFe2As2 results, there is no measurable Meissner effect and no suppression of the resistive superconducting transition with annealing. The current sensitivity of the superconducting resistive transition in our samples of BaFe2As2 is quite strong, with an increase in the current density of a factor of 15 to ~ 1.5 A/cm2 not changing Tc(onset) but broadening the transition significantly and causing the resistivity to remain finite as T approaches 0. To investigate if this unusually low critical current is indicative of filamentary conduction lacking the apparent anisotropy seen in the critical magnetic field, Hc2, measurements of, e. g., the bulk superconductor Co-doped BaFe2As2, Hc2 was measured in both crystalline directions. These BaFe2As2 samples show Hc2(T) values in the ab-plane and along the c-axis comparable to those seen in BaFe2-xCoxAs2, which has a similar Tc. Since the lack of Tc suppression after annealing argues against strain-induced superconductivity as proposed for the other undoped MFe2As2 materials, another possible cause for the superconductivity in BaFe2As2 is discussed.",0907.4429v1 2019-03-12,Signatures of Anelastic Domain Relaxation in Ba(Fe$_{1-x}$Co$_{x}$)$_{2}$As$_{2}$ Investigated by Mechanical Modulation of Resistivity,"The resistive response of Ba(Fe$_{1-x}$Co$_{x}$)$_{2}$As$_{2}$ to AC mechanical deformation is considered in the multi-domain state. This resistance change depends both upon the anelastic relaxation of domain walls and upon the relation between resistance and the domain wall configuration. Samples are adhered to the surface of a piezoelectric stack, which is driven by an AC voltage while the AC modulation of the sample resistance is measured. As the response time of electrons is faster than that of the lattice, the phase difference $\phi$ between the AC resistance modulation and the AC deformation of the piezoelectric is entirely due to anelastic relaxation effects in the sample. An expression is derived for relating $\phi$ to a sample's complex compliance, $J(\omega)$, in this experimental configuration. Measurements of Ba(Fe$_{1-x}$Co$_{x}$)$_{2}$As$_{2}$ for x= (0.025, 0.052) reveal a peak in the out-of-phase resistivity modulation in the orthorhombic antiferromagnetic state well below the Ne\'el temperature $T_N$ and structural transition $T_S$. Meanwhile, for a composition that is tetragonal at all temperatures, x=0.07, the resistance modulation remains entirely in phase over the same temperatures, establishing domain motion as a probable cause of the observed effects in the samples that do undergo the tetragonal-to-orthorhombic transition. Fits are provided of $\tan\phi$ for a sample with x=0.025 for various amplitude excitations on the piezoelectric stack, from which the apparent activation energy $E_a$ for domain wall motion is found to decreases with increasing amplitude of the deformation along the $[110]_T$ axis. We find $\frac{dE_a}{d\varepsilon^0_{[110,110]_T}} = -1115\pm 196$ eV with $E_a = 9.09 \pm 0.74 \times 10^{-3}$ eV in the zero strain limit if we assume linearity over the entire range of strain amplitudes.",1903.04732v1 2005-02-09,"Structure, magnetic and transport properties of Ti-substituted La0.7Sr0.3MnO3","Ti-substituted perovskites, La0.7Sr0.3Mn1-xTixO3, with x between 0 to 0.20, were investigated by neutron diffraction, magnetization, electric resistivity, and magnetoresistance (MR) measurements. All samples show a rhombohedral structure (space group R3c) from 10 K to room temperature. At room temperature, the cell parameters a, c and the unit cell volume increase with increasing Ti content. However, at 10 K, the cell parameter a has a maximum value for x = 0.10, and decreases for x greater than 0.10, while the unit cell volume remains nearly constant for x greater than 0.10. The average (Mn,Ti)-O bond length increases up to x=0.15, and the (Mn,Ti)-O-(Mn,Ti) bond angle decreases with increasing Ti content to its minimum value at x=0.15 at room temperature. Below the Curie temperature T_C, the resistance exhibits metallic behavior for the x _ 0.05 samples. A metal (semiconductor) to insulator transition is observed for the x_ 0.10 samples. A peak in resistivity appears below T_C for all samples, and shifts to a lower temperature as x increases. The substitution of Mn by Ti decreases the 2p-3d hybridization between O and Mn ions, reduces the bandwidth W, and increases the electron-phonon coupling. Therefore, the TC shifts to a lower temperature and the resistivity increases with increasing Ti content. A field-induced shift of the resistivity maximum occurs at x less than or equal to 0.10. The maximum MR effect is about 70% for La0.7Sr0.3Mn0.8Ti0.2O3. The separation of TC and the resistivity maximum temperature Tmax enhances the MR effect in these compounds due to the weak coupling between the magnetic ordering and the resistivity as compared with La0.7Sr0.3MnO3.",0502235v1 2020-12-08,Quantitative measurement of the thermal contact resistance between a glass microsphere and a plate,"Accurate measurements of the thermal resistance between micro-objects made of insulating materials are complex because of their small size, low conductivity, and the presence of various ill-defined gaps. We address this issue using a modified scanning thermal microscope operating in vacuum and in air. The sphere-plate geometry is considered. Under controlled heating power, we measure the temperature on top of a glass microsphere glued to the probe as it approaches a glass plate at room temperature with nanometer accuracy. In vacuum, a jump is observed at contact. From this jump in temperature and the modeling of the thermal resistance of a sphere, the sphere-plate contact resistance $ R_K=(1.4 \pm 0.18)\times10^7 \ \mathrm{K.W^{-1}}$ and effective radius $r=(36 \pm 4)$ nm are obtained. In air, the temperature on top of the sphere shows a decrease starting from a sphere-plate distance of 200 $\mathrm{\mu m}$. A jump is also observed at contact, with a reduced amplitude. The sphere-plate coupling out of contact can be described by the resistance shape factor of a sphere in front of a plate in air, placed in a circuit involving a series and a parallel resistance that are determined by fitting the approach curve. The contact resistance in air $R^*_K=(1.2 \pm 0.46)\times 10^7 \ \mathrm{K.W^{-1}}$ is then estimated from the temperature jump. The method is quantitative without requiring any tedious multiple-scale numerical simulation, and is versatile to describe the coupling between micro-objects from large distances to contact in various environments.",2012.04291v1 2002-01-19,Antiferromagnetic Order Induced by an Applied Magnetic Field in a High-Temperature Superconductor,"One view of the cuprate high-transition temperature (high-Tc) superconductors is that they are conventional superconductors where the pairing occurs between weakly interacting quasiparticles, which stand in one-to-one correspondence with the electrons in ordinary metals - although the theory has to be pushed to its limit. An alternative view is that the electrons organize into collective textures (e.g. charge and spin stripes) which cannot be mapped onto the electrons in ordinary metals. The phase diagram, a complex function of various parameters (temperature, doping and magnetic field), should then be approached using quantum field theories of objects such as textures and strings, rather than point-like electrons. In an external magnetic field, magnetic flux penetrates type-II superconductors via vortices, each carrying one flux quantum. The vortices form lattices of resistive material embedded in the non-resistive superconductor and can reveal the nature of the ground state - e.g. a conventional metal or an ordered, striped phase - which would have appeared had superconductivity not intervened. Knowledge of this ground state clearly provides the most appropriate starting point for a pairing theory. Here we report that for one high-Tc superconductor, the applied field which imposes the vortex lattice, also induces antiferromagnetic order. Ordinary quasiparticle pictures cannot account for the nearly field-independent antiferromagnetic transition temperature revealed by our measurements.",0201349v1 2013-01-22,Exceptional ballistic transport in epitaxial graphene nanoribbons,"Graphene electronics has motivated much of graphene science for the past decade. A primary goal was to develop high mobility semiconducting graphene with a band gap that is large enough for high performance applications. Graphene ribbons were thought to be semiconductors with these properties, however efforts to produce ribbons with useful bandgaps and high mobility has had limited success. We show here that high quality epitaxial graphene nanoribbons 40 nm in width, with annealed edges, grown on sidewall SiC are not semiconductors, but single channel room temperature ballistic conductors for lengths up to at least 16 micrometers. Mobilities exceeding one million corresponding to a sheet resistance below 1 Ohm have been observed, thereby surpassing two dimensional graphene by 3 orders of magnitude and theoretical predictions for perfect graphene by more than a factor of 10. The graphene ribbons behave as electronic waveguides or quantum dots. We show that transport in these ribbons is dominated by two components of the ground state transverse waveguide mode, one that is ballistic and temperature independent, and a second thermally activated component that appears to be ballistic at room temperature and insulating at cryogenic temperatures. At room temperature the resistance of both components abruptly increases with increasing length, one at a length of 160 nm and the other at 16 micrometers. These properties appear to be related to the lowest energy quantum states in the charge neutral ribbons. Since epitaxial graphene nanoribbons are readily produced by the thousands, their room temperature ballistic transport properties can be used in advanced nanoelectronics as well.",1301.5354v2 2022-01-25,KCo$_2$As$_2$: A New Portal for the Physics of High-Purity Metals,"High-quality single crystals of KCo$_2$As$_2$ with the body-centered tetragonal ThCr$_2$Si$_2$ structure were grown using KAs self flux. Structural, magnetic, thermal, and electrical transport were investigated. No clear evidence for any phase transitions was found in the temperature range 2 to 300 K. The in-plane electrical resistivity $\rho$ versus temperature $T$ is highly unusual, showing a $T^4$ behavior below 30 K and an anomalous positive curvature up to 300 K which is different from the linear behavior expected from the Bloch-Gr\""uneisen theory for electron scattering by acoustic phonons. This positive curvature has been previously observed in the in-plane resistivity of high-conductivity layered delafossites such as PdCoO$_2$ and PtCoO$_2$. The in-plane $\rho(T\to0) = 0.36~\mu\Omega$ cm of KCo$_2$As$_2$ is exceptionally small for this class of compounds. The material also exhibits a nearly linear magnetoresistance at low $T$ which attains a value of about 40% at $T=2$K and magnetic field $H= 80$ kOe. The magnetic susceptibility $\chi$ of KCo$_2$As$_2$ is isotropic and about an order of magnitude smaller than the values for the related compounds SrCo$_2$As$_2$ and BaCo$_2$As$_2$. The $\chi$ increases above 100 K which is found from our first-principles calculations to arise from a sharp peak in the electronic density of states just above the Fermi energy $E_{\rm F}$. Heat capacity $C_{\rm p}(T)$ data at low $T$ yield an electronic density of states $N(E_{\rm F})$ that is about 36% larger than predicted by the first-principles theory. The $C_{\rm p}(T)$ data near room temperature suggest the presence of excited optic vibration modes which may also be the source of the positive curvature in $\rho(T)$. Our results show that KCo$_2$As$_2$ provides a new avenue for investigating the physics of high-purity metals.",2201.10325v1 2023-01-25,Investigation of Planckian behavior in a high-conductivity oxide: PdCrO$_2$,"The layered delafossite metal PdCrO$_2$ is a natural heterostructure of highly conductive Pd layers Kondo coupled to localized spins in the adjacent Mott insulating CrO$_2$ layers. At high temperatures $T$ it has a $T$-linear resistivity which is not seen in the isostructural but non-magnetic PdCoO$_2$. The strength of the Kondo coupling is known, as-grown crystals are extremely high purity and the Fermi surface is both very simple and experimentally known. It is therefore an ideal material platform in which to investigate 'Planckian metal' physics. We do this by means of controlled introduction of point disorder, measurement of the thermal conductivity and Lorenz ratio and studying the sources of its high temperature entropy. The $T$-linear resistivity is seen to be due mainly to elastic scattering and to arise from a sum of several scattering mechanisms. Remarkably, this sum leads to a scattering rate within 10$\%$ of the Planckian value of $k_BT/$$\hbar$.",2301.10631v1 1995-06-01,Role of phason-defects on the conductance of a 1-d quasicrystal,"We have studied the influence of a particular kind of phason-defect on the Landauer resistance of a Fibonacci chain. Depending on parameters, we sometimes find the resistance to decrease upon introduction of defect or temperature, a behavior that also appears in real quasicrystalline materials. We demonstrate essential differences between a standard tight-binding model and a full continuous model. In the continuous case, we study the conductance in relation to the underlying chaotic map and its invariant. Close to conducting points, where the invariant vanishes, and in the majority of cases studied, the resistance is found to decrease upon introduction of a defect. Subtle interference effects between a sudden phason-change in the structure and the phase of the wavefunction are also found, and these give rise to resistive behaviors that produce exceedingly simple and regular patterns.",9506004v2 1997-12-12,Surface Resistance Imaging with a Scanning Near-Field Microwave Microscope,"We describe near-field imaging of sample sheet resistance via frequency shifts in a resonant coaxial scanning microwave microscope. The frequency shifts are related to local sample properties, such as surface resistance and dielectric constant. We use a feedback circuit to track a given resonant frequency, allowing measurements with a sensitivity to frequency shifts as small as one parts in 50000 for a 30 ms sampling time. The frequency shifts can be converted to sheet resistance based on a simple model of the system.",9712142v1 1997-12-15,Quantitative Imaging of Sheet Resistance with a Scanning Near-Field Microwave Microscope,"We describe quantitative imaging of the sheet resistance of metallic thin films by monitoring frequency shift and quality factor in a resonant scanning near-field microwave microscope. This technique allows fast acquisition of images at approximately 10 ms per pixel over a frequency range from 0.1 to 50 GHz. In its current configuration, the system can resolve changes in sheet resistance as small as 0.6 Ohms/sq for 100 Ohms/sq films. We demonstrate its use at 7.5 GHz by generating a quantitative sheet resistance image of a YBa2Cu3O7 (YBCO) thin film on a 5 cm-diameter sapphire wafer.",9712171v1 1999-07-13,Na-site substitution effects of the thermoelectric properties of NaCo_2O_4,"The resistivity and thermopower of Na$_{1+x}$Co$_2$O$_4$ and Na$_{1.1-x}$Ca$_x$Co$_2$O$_4$ are measured and analyzed. In Na$_{1+x}$Co$_2$O$_4$, whereas the resistivity increases with $x$, the thermopower is nearly independent of $x$. This suggests that the excess Na is unlikely to supply carriers, and decreases effective conduction paths in the sample. In Na$_{1.1-x}$Ca$_x$Co$_2$O$_4$, the resistivity and the thermopower increase with $x$, and the Ca$^{2+}$ substitution for Na$^+$ reduces the majority carriers in NaCo$_2$O$_4$. This means that they are holes, which is consistent with the positive sign of the thermopower. Strong correlation in this compound is evidenced by the peculiar temperature dependence of the resistivity.",9907179v1 1999-11-06,Electrical Resistivity of a Thin Metallic Film,"The electrical resistivity of a pure sample of a thin metallic film is found to depend on the boundary conditions. This conclusion is supported by a free-electron model calculation and confirmed by an ab initio relativistic Korringa-Kohn-Rostoker computation. The low-temperature resistivity is found to be zero for a free-standing film (reflecting boundary conditions) but nonzero when the film is sandwiched between two semi-infinite samples of the same material (outgoing boundary conditions). In the latter case, this resistivity scales inversely with the number of monolayers and is due to the background diffusive scattering by a finite lattice.",9911093v1 2000-03-09,On the Mooij Rule,"Weak localization leads to the same correction to both the conductivity and the electron-phonon coupling constant $\lambda$ (and $\lambda_{tr}$). Consequently the temperature dependence of the (thermal) electrical resistivity is decreasing as the conductivity is decreasing due to weak localization, which results in the decrease of the temperature coefficient of resistivity (TCR) with increasing the residual resistivity. When $\lambda$ is approaching zero, only residual resistivity part remains and gives rise to the negative TCR. Accordingly, the Mooij rule is a manifestation of weak localization correction to the conductivity and the electron-phonon interaction. This study may provide a new means of probing the phonon-mechanism in exotic superconductors.",0003144v1 2001-05-04,Weak localization and the Mooij rule in disordered metals,"Weak localization leads to the same correction to both the conductivity and the McMillan's electron-phonon coupling constant $\lambda$ (and $\lambda_{tr}$). Consequently the temperature dependence of the thermal electrical resistivity is decreasing as the conductivity is decreasing due to weak localization, which results in the decrease of the temperature coefficient of resistivity (TCR) with increasing the residual resistivity. When $\lambda$ and $\lambda_{tr}$ are approaching zero, only residual resistivity part remains and gives rise to the negative TCR. Accordingly, the Mooij rule is a manifestation of weak localization correction to the conductivity and the electron-phonon interaction. This study may provide a new means of probing the phonon-mechanism in exotic superconductors.",0105090v1 2001-10-31,Stationary Regime of Random Resistor Networks Under Biased Percolation,"The state of a 2-D random resistor network, resulting from the simultaneous evolutions of two competing biased percolations, is studied in a wide range of bias values. Monte Carlo simulations show that when the external current $I$ is below the threshold value for electrical breakdown, the network reaches a steady state with a nonlinear current-voltage characteristic. The properties of this nonlinear regime are investigated as a function of different model parameters. A scaling relation is found between $/_0$ and $I/I_0$, where $$ is the average resistance, $_0$ the linear regime resistance and $I_0$ the threshold value for the onset of nonlinearity. The scaling exponent is found to be independent of the model parameters. A similar scaling behavior is also found for the relative variance of resistance fluctuations. These results compare well with resistance measurements in composite materials performed in the Joule regime up to breakdown.",0110646v1 2002-05-27,Resistivity and thermoelectric power measurements on CeFe$_2$ and its pseudobinaries,"Resistivity and thermoelectric power (TEP) measurements on CeFe$_2$ and two of its pseudo-binaries Ce(Fe, 5% Ir)$_2$ and Ce(Fe, 7% Ru)$_2$ between 78K and 275K are reported. The resistivity data are analysed in terms of contributions from scattering due to phonon, magnon, spin fluctuation and lattice defects, and also from interband scattering. Attempts are made to analyze the TEP data in terms of these resistivity components. Thermal hysteresis is observed in the temperature dependence of TEP in the Ir and Ru doped CeFe$_2$ samples around the ferromagnetic to antiferromagnetic transition, indicating the first order nature of this transition.",0205539v1 2003-02-12,Temperature Dependence of the Dielectric Constant and Resistivity of Diluted Magnetic Semiconductors,"We study the effect that the ferromagnetic order has on the electrical properties of Diluted Magnetic Semiconductors. We analyze the temperature dependence of the dielectric constant and of the resistivity of Ga$_{1-x}$Mn$_x$As. In our treatment the electronic structure of the semiconductor is described by a six band Kohn-Luttinger Hamiltonian, the thermal fluctuations of the Mn magnetic moments are treated in the mean field approximation, the carrier-carrier interaction within the random phase approximation, and the transport properties using the relaxation time approximation. We find that the Thomas-Fermi length changes near 8% when going from the ferromagnetic to the paramagnetic phase. We also find, in good agreement with the experiments, that the resistivity changes near 20% when going from zero to the Curie temperature. We explain this change in the resistivity in terms of the variation of the Fermi surface and the transport scattering time when going from the ferromagnetic phase to the paramagnetic phase.",0302237v1 2003-02-19,Small-polaron hopping conductivity in bilayer manganite La$_{1.2}$Sr$_{1.8}$Mn$_{2}$O$_{7}$,"We report anisotropic resistivity measurements on a La$_{1.2}$Sr$_{1.8}$Mn$_{2}$O$_{7}$ single crystal over a temperature $T$ range from 2 to 400 K and in magnetic fields $H$ up to 14 T. For $T\geq 218$ K, the temperature dependence of the zero-field in-plane $\rho_{ab}(T)$ resistivity obeys the adiabatic small polaron hopping mechanism, while the out-of-plane $\rho_{c}(T)$ resistivity can be ascribed by an Arrhenius law with the same activation energy. Considering the magnetic character of the polarons and the close correlation between the resistivity and magnetization, we developed a model which allows the determination of $\rho_{ab,c}(H,T)$. The excellent agreement of the calculations with the measurements indicates that small polarons play an essential role in the electrical transport properties in the paramagnetic phase of bilayer manganites.",0302392v1 2003-07-21,Detecting percolative metal-insulator transition in manganites by resistive relaxation,"We report an experimental study of the time dependence of resistivity of a La$_{0.9}$Sr$_{0.1}$MnO$_{3}$ ultrathin film in order to elucidate the underlying mechanism for metal-insulator transition and colossal magnetoresistance CMR effect. There is a clear change of sign in the resistive relaxation rate across the metal-insulator transition driven by temperature or magnetic field. When measuring in increasing temperature or decreasing magnetic field, the resistivity increases with time in the metallic state but decreases with time in the insulating state. These relaxation processes indicate that the metal-insulator transition and the associated CMR are a direct result of phase separation and of percolation of the metallic phase.",0307501v1 2004-11-24,Electrical Spin Injection in Multi-Wall carbon NanoTubes with transparent ferromagnetic contacts,"We report on electrical spin injection measurements on MWNTs . We use a ferromagnetic alloy Pd$_{1-x}$Ni$_{x}$ with x $\approx$ 0.7 which allows to obtain devices with resistances as low as 5.6 $k\Omega$ at 300 $K$. The yield of device resistances below 100 $k\Omega$, at 300 $K$, is around 50%. We measure at 2 $K$ a hysteretic magneto-resistance due to the magnetization reversal of the ferromagnetic leads. The relative difference between the resistance in the antiparallel (AP) orientation and the parallel (P) orientation is about 2%.",0411623v2 2005-04-22,Possible Localization Behavior of the Inherent Conducting Polymer (CH$_3$)$_{0.9}$ReO$_3$,"Polymeric methyltrioxorhenium (poly-MTO) represents the first example of an inherent conducting organometallic oxide. It adopts the structural motives and transport properties of some classical perovskites in two dimensions. In this study we present resistivity data down to 30 mK which exhibit a crossover from a metallic (d$\rho$/d$T >$ 0) to an insulating (d$\rho$/d$T <$ 0) behavior at about 30 K. Below 30 K an unusual resistivity behavior, similar to that of some doped cuprate systems, is observed: initially the resistivity increases approximately as $\rho \sim$ log$(1/T$) before it starts to saturate below 2 K. Furthermore, a linear positive magnetoresistance is found (up to 7 T). Temperature dependent magnetization and specific heat measurements in various magnetic fields indicate that the unusual resistivity behavior may be driven by spatial localization of the d$^1$ moments at the Re atoms.",0504585v1 2005-04-27,Colossal resistivity change besides magnetoresistance: an extended theoretical framework for electronic transport of manganites,"Current theoretical approaches to manganites mainly stem from magnetic framework, in which the electronic transport is thought to be spin-dependent and the double exchange mechanism plays a core role. However, quite a number of experimental observations can yet not be reasonably explained. For example, multiplicate insulator-metal transitions and resistivity reduction induced by perturbations other than magnetic field, such as electric current, are not well understood. A comprehensive analysis on earlier extensive studies is performed and two types of origins for resistivity change are highlighted. Besides the insulated-to-metallic transition induced by external field such as magnetic field, the insulated-to-insulated transition induced extrinsically is even a more important source for the colossal resistivity change. We propose an extended framework for the electronic transport of manganites, in which the contribution of charge degree of freedom is given a special priority.",0504706v2 2006-01-31,Phase coexistence and resistivity near the ferromagnetic transition of manganites,"Pairing of oxygen holes into heavy bipolarons in the paramagnetic phase and their magnetic pair-breaking in the ferromagnetic phase [the so-called current-carrier density collapse (CCDC)] has accounted for the first-order ferromagnetic phase transition, colossal magnetoresistance (CMR), isotope effect, and pseudogap in doped manganites. Here we propose an explanation of the phase coexistence and describe the magnetization and resistivity of manganites near the ferromagnetic transition in the framework of CCDC. The present quantitative description of resistivity is obtained without any fitting parameters by using the experimental resistivities far away from the transition and the experimental magnetization, and essentially model independent.",0601712v2 2006-02-03,Boundary resistance in magnetic multilayers,"Quasiclassical boundary conditions for electrochemical potentials at the interface between diffusive ferromagnetic and non-magnetic metals are derived for the first time. An expression for the boundary resistance accurately accounts for the momentum conservation law as well as essential gradients of the chemical potentials. Conditions are established at which spin-asymmetry of the boundary resistance has positive or negative sign. Dependence of the spin asymmetry and the absolute value of the boundary resistance on the exchange splitting of the conduction band opens up new possibility to estimate spin polarization of the conduction band of ferromagnetic metals. Consistency of the theory is checked on existing experimental data.",0602070v1 2006-06-23,Angular dependence of domain wall resistivity in artificial magnetic domain structures,"We exploit the ability to precisely control the magnetic domain structure of perpendicularly magnetized Pt/Co/Pt trilayers to fabricate artificial domain wall arrays and study their transport properties. The scaling behaviour of this model system confirms the intrinsic domain wall origin of the magnetoresistance, and systematic studies using domains patterned at various angles to the current flow are excellently described by an angular-dependent resistivity tensor containing perpendicular and parallel domain wall resistivities. We find that the latter are fully consistent with Levy-Zhang theory, which allows us to estimate the ratio of minority to majority spin carrier resistivities, rho-down/rho-up~5.5, in good agreement with thin film band structure calculations.",0606614v1 2006-07-26,"Angle-dependent magnetotransport in cubic and tetragonal ferromagnets: Application to (001)- and (113)A-oriented (Ga,Mn)As","General expressions for the longitudinal and transverse resistivities of single-crystalline cubic and tetragonal ferromagnets are derived from a series expansion of the resistivity tensor with respect to the magnetization orientation. They are applied to strained (Ga,Mn)As films, grown on (001)- and (113)A-oriented GaAs substrates, where the resistivities are theoretically and experimentally studied for magnetic fields rotated within various planes parallel and perpendicular to the sample surface. We are able to model the measured angular dependences of the resistivities within the framework of a single ferromagnetic domain, calculating the field-dependent orientation of the magnetization by numerically minimizing the free-enthalpy density. Angle-dependent magnetotransport measurements are shown to be a powerful tool for probing both anisotropic magnetoresistance and magnetic anisotropy. The anisotropy parameters of the (Ga,Mn)As films inferred from the magnetotransport measurements agree with those obtained by ferromagnetic resonance measurements within a factor of two.",0607679v1 2006-11-14,Calculations of spin-disorder resistivity from first principles,"Spin-disorder resistivity of Fe and Ni is studied using the noncollinear density functional theory. The Landauer conductance is averaged over random disorder configurations and fitted to Ohm's law. The distribution function is approximated by the mean-field theory. The dependence of spin-disorder resistivity on magnetization in Fe is found to be in excellent agreement with the results for the isotropic s-d model. In the fully disordered state, spin-disorder resistivity for Fe is close to experiment, while for fcc Ni it exceeds the experimental value by a factor of 2.3. This result indicates strong magnetic short-range order in Ni at the Curie temperature.",0611377v2 2007-04-04,Vortex Dynamics at the Initial Stage of Resistive Transition in Superconductors with Fractal Cluster Structure,"The effect of fractal normal-phase clusters on vortex dynamics in a percolative superconductor is considered. The superconductor contains percolative superconducting cluster carrying a transport current and clusters of a normal phase, acting as pinning centers. A prototype of such a structure is YBCO film, containing clusters of columnar defects, as well as the BSCCO/Ag sheathed tape, which is of practical interest for wire fabrication. Transition of the superconductor into a resistive state corresponds to the percolation transition from a pinned vortex state to a resistive state when the vortices are free to move. The dependencies of the free vortex density on the fractal dimension of the cluster boundary as well as the resistance on the transport current are obtained. It is revealed that a mixed state of the vortex glass type is realized in the superconducting system involved. The current-voltage characteristics of superconductors containing fractal clusters are obtained and their features are studied.",0704.0494v1 2008-02-19,Temperature memory and resistive glassy behaviors of a perovskite manganite,"This paper reports the observations of long-time relaxation, aging, and temperature memory behaviors of resistance and magnetization in the ferromagnetic state of a polycrystalline La0.7Ca0.3Mn0.925Ti0.075O3 compound. The observed glassy dynamics of the electrical transport appears to be magnetically originated and has a very close association with the magnetic glassiness of the sample. Phase separation and strong correlation between magnetic interactions and electronic conduction play the essential roles in producing such a resistive glassiness. We explain the observed effects in terms of a coexistence of two competing thermomagnetic processes, domain growth and magnetic freezing, and propose that hole-doped perovskite manganites can be considered as ""resistive glasses"".",0802.2729v1 2008-02-26,Effects of heat dissipation on unipolar resistance switching in Pt/NiO/Pt capacitors,"We fabricated Pt/NiO/Pt capacitor structures with various bottom electrode thicknesses, $t_{BE}$, and investigated their resistance switching behaviors. The capacitors with $t_{BE} \geq 50$ nm exhibited typical unipolar resistance memory switching, while those with $t_{BE} \leq 30$ nm showed threshold switching. This interesting phenomenon can be explained in terms of the temperature-dependent stability of conducting filaments. In particular, the thinner $t_{BE}$ makes dissipation of Joule heat less efficient, so the filaments will be at a higher temperature and become less stable. This study demonstrates the importance of heat dissipation in resistance random access memory.",0802.3739v1 2008-08-25,Stability and normal zone propagation speed in YBCO coated conductors with increased interfacial resistance,"We will discuss how stability and speed of normal zone propagation in YBCO-coated conductors is affected by interfacial resistance between the superconducting film and the stabilizer. Our numerical simulation has shown that the increased interfacial resistance substantially increases speed of normal zone propagation and decreases the stability margins. Optimization of the value of the resistance may lead to a better compromise between stability and quench protection requirements than what is found in currently manufactured coated conductors.",0808.3409v3 2008-12-12,Magnetic tunnel junctions with ferroelectric barriers: Prediction of four resistance states from first-principles,"Magnetic tunnel junctions (MTJs), composed of two ferromagnetic electrodes separated by a thin insulating barrier layer, are currently used in spintronic devices, such as magnetic sensors and magnetic random access memories. Recently, driven by demonstrations of ferroelectricity at the nanoscale, thin-film ferroelectric barriers were proposed to extend the functionality of MTJs. Due to the sensitivity of conductance to the magnetization alignment of the electrodes (tunnelling magnetoresistance) and the polarization orientation in the ferroelectric barrier (tunnelling electroresistance), these multiferroic tunnel junctions (MFTJs) may serve as four-state resistance devices. Based on first-principles calculations we demonstrate four resistance states in SrRuO3/BaTiO3/SrRuO3 MFTJs with asymmetric interfaces. We find that the resistance of such a MFTJ is significantly changed when the electric polarization of the barrier is reversed and/or when the magnetizations of the electrodes are switched from parallel to antiparallel. These results reveal the exciting prospects of MFTJs for application as multifunctional spintronic devices.",0812.2393v1 2008-12-23,Specific Resistance of Pd/Ir Interfaces,"From measurements of the current-perpendicular-to-plane (CPP) total specific resistance (AR = area times resistance) of sputtered Pd/Ir multilayers, we derive the interface specific resistance, 2AR(Pd/Ir) = 1.02 +/- 0.06 fOhmm^2, for this metal pair with closely similar lattice parameters. Assuming a single fcc crystal structure with the average lattice parameter, no-free-parameter calculations, including only spd orbitals, give for perfect interfaces, 2AR(Pd/Ir)(Perf) = 1.21 +/-0.1 fOhmm^2, and for interfaces composed of two monolayers of a random 50%-50% alloy, 2AR(Pd/Ir)(50/50) = 1.22 +/- 0.1 fOhmm^2. Within mutual uncertainties, these values fall just outside the range of the experimental value. Updating to add f-orbitals gives 2AR(Pd/Ir)(Perf) = 1.10 +/- 0.1 fOhmm^2 and 2AR(Pd/Ir)(50-50) = 1.13 +/- 0.1 fOhmm^2, values now compatible with the experimental one. We also update, with f-orbitals, calculations for other pairs",0812.4421v1 2010-01-11,Anomalous Hall Effect in Fe/Gd Bilayers,"Non-monotonic dependence of anomalous Hall resistivity on temperature and magnetization, including a sign change, was observed in Fe/Gd bilayers. To understand the intriguing observations, we fabricated the Fe/Gd bilayers and single layers of Fe and Gd simultaneously. The temperature and field dependences of longitudinal resistivity, Hall resistivity and magnetization in these films have also been carefully measured. The analysis of these data reveals that these intriguing features are due to the opposite signs of Hall resistivity/or spin polarization and different Curie temperatures of Fe and Gd single-layer films.",1001.1586v2 2010-10-26,Evanescent incompressible strips as origin of the observed Hall resistance overshoot,"In this work we provide a systematic explanation to the unusual non-monotonic behavior of the Hall resistance observed at two-dimensional electron systems. We use a semi-analytical model based on the interaction theory of the integer quantized Hall effect to investigate the existence of the anomalous, \emph{i.e} overshoot, Hall resistance $R_{H}$. The observation of the overshoot resistance at low magnetic field edge of the plateaus is elucidated by means of overlapping evanescent incompressible strips, formed due to strong magnetic fields and interactions. Utilizing a self-consistent numerical scheme we also show that, if the magnetic field is decreased the $R_{H}$ decreases to its expected value. The effects of the sample width, temperature, disorder strength and magnetic field on the overshoot peaks are investigated in detail. Based on our findings, we predict a controllable procedure to manipulate the maxima of the peaks, which can be tested experimentally. Our model does not depend on specific and intrinsic properties of the material, provided that a single particle gap exists.",1010.5432v1 2010-12-13,Distinct electronic nematicities between electron and hole underdoped iron pnictides,"We systematically investigated the in-plane resistivity anisotropy of electron-underdoped $EuFe_{2-x}Co_xAs_2$ and $BaFe_{2-x}Co_xAs_2$, and hole-underdoped $Ba_{1-x}K_xFe_2As_2$. Large in-plane resistivity anisotropy was found in the former samples, while {\it tiny} in-plane resistivity anisotropy was detected in the latter ones. When it is detected, the anisotropy starts above the structural transition temperature and increases smoothly through it. As the temperature is lowered further, the anisotropy takes a dramatic enhancement through the magnetic transition temperature. We found that the anisotropy is universally tied to the presence of non-Fermi liquid T-linear behavior of resistivity. Our results demonstrate that the nematic state is caused by electronic degrees of freedom, and the microscopic orbital involvement in magnetically ordered state must be fundamentally different between the hole and electron doped materials.",1012.2731v1 2011-01-31,Phase Mixing of Nonlinear Visco-resistive Alfvén Waves,"We investigate the behaviour of nonlinear, nonideal Alfv\'en wave propagation within an inhomogeneous magnetic environment. The governing MHD equations are solved in 1D and 2D using both analytical techniques and numerical simulations. We find clear evidence for the ponderomotive effect and visco-resistive heating. The ponderomotive effect generates a longitudinal component to the transverse Alfv\'en wave, with a frequency twice that of the driving frequency. Analytical work shows the addition of resistive heating. This leads to a substantial increase in the local temperature and thus gas pressure of the plasma, resulting in material being pushed along the magnetic field. In 2D, our system exhibits phase mixing and we observe an evolution in the location of the maximum heating, i.e. we find a drifting of the heating layer. Considering Alfv\'en wave propagation in 2D with an inhomogeneous density gradient, we find that the equilibrium density profile is significantly modified by both the flow of density due to visco-resistive heating and the nonlinear response to the localised heating through phase mixing.",1101.5945v1 2011-03-04,Voltage bias induced modification of all oxide Pr0.5Ca0.5MnO3/SrTi0.95Nb.05O3 junctions,"In this paper we report what happens to a pristine oxide junction Pr0.5Ca0.5MnO3/SrTi0.95Nb.05O3 (PCMO/Nb:STO), when it is subjected to cycling of voltage bias of moderate value ({\pm}4V). It is found that the initial cycling leads to formation of a permanent state of lower resistance where the lower resistance arises predominantly due to development of a shunt across the device film (PCMO). On successive voltage cycling with increasing magnitude, this state transforms into states of successive lower resistance that can be transformed back to the initial stable state on cycling to below a certain bias. A simple model based on p-n junction with shunt has been used to obtain information on the change of the junction on voltage cycling. It has been shown that the observation can be explained if the voltage cycling leads to lowering of barrier at the interface and also reduction in series resistance. It is suggested that this lowering can be related to the migration of oxygen ions and vacancies at the junction region. Cross-sectional imaging of the junction shows formation of permanent filamentary bridges across the thickness of the PCMO after the pristine p-n junction is first taken through a voltage cycle, which would explain appearance of a finite shunt across the p-n junction.",1103.0884v1 2011-07-11,Magnetotransport properties of iron microwires fabricated by focused electron beam induced autocatalytic growth,"We have prepared iron microwires in a combination of focused electron beam induced deposition (FEBID) and autocatalytic growth from the iron pentacarbonyl, Fe(CO)5, precursor gas under UHV conditions. The electrical transport properties of the microwires were investigated and it was found that the temperature dependence of the longitudinal resistivity (rhoxx) shows a typical metallic behaviour with a room temperature value of about 88 micro{\Omega} cm. In order to investigate the magnetotransport properties we have measured the isothermal Hall-resistivities in the range between 4.2 K and 260 K. From these measurements positive values for the ordinary and the anomalous Hall coefficients were derived. The relation between anomalous Hall resistivity (rhoAN) and longitudinal resistivity is quadratic, rhoAN rho^2 xx, revealing an intrinsic origin of the anomalous Hall effect. Finally, at low temperature in the transversal geometry a negative magnetoresistance of about 0.2 % was measured.",1107.2014v1 2011-08-11,Effect of Electron-electron Interaction on Surface Transport in Three-Dimensional Topological Insulators,"We study the effect of electron-electron interaction on the surface resistivity of three-dimensional (3D) topological insulators. In the absence of umklapp scattering, the existence of the Fermi-liquid ($T^2$) term in resistivity of a two-dimensional (2D) metal depends on the Fermi surface geometry, in particular, on whether it is convex or concave. On doping, the Fermi surface of 2D metallic surface states in 3D topological insulators of the Bi$_2$Te$_3$ family changes its shape from convex to concave due to hexagonal warping, while still being too small to allow for umklapp scattering. We show that the $T^2$ term in the resistivity is present only in the concave regime and demonstrate that the resistivity obeys a universal scaling form valid for an arbitrary 2D Fermi surface near a convex/concave transition.",1108.2435v1 2011-10-31,Spin Transfer from a Ferromagnet into a Semiconductor through an Oxide barrier,"We present results on the magnetoresistance of the system Ni/Al203/n-doped Si/Al2O3/Ni in fabricated nanostructures. The results at temperature of 14K reveal a 75% magnetoresistance that decreases in value up to approximately 30K where the effect disappears. We observe minimum resistance in the antiparallel configurations of the source and drain of Ni. As a possibility, it seems to indicate the existence of a magnetic state at the Si/oxide interface. The average spin diffusion length obtained is of 650 nm approximately. Results are compared to the window of resistances that seems to exist between the tunnel barrier resistance and two threshold resistances but the spin transfer seems to work in the range and outside the two thresholds.",1110.6810v1 2012-08-22,Why is the bulk resistivity of topological insulators so small?,"As-grown topological insulators (TIs) are typically heavily-doped $n$-type crystals. Compensation by acceptors is used to move the Fermi level to the middle of the band gap, but even then TIs have a frustratingly small bulk resistivity. We show that this small resistivity is the result of band bending by poorly screened fluctuations in the random Coulomb potential. Using numerical simulations of a completely compensated TI, we find that the bulk resistivity has an activation energy of just 0.15 times the band gap, in good agreement with experimental data. At lower temperatures activated transport crosses over to variable range hopping with a relatively large localization length.",1208.4601v2 2012-09-26,Substrate effect on the resistive switching in BiFeO3 thin films,"BiFeO3 thin films have been deposited on Pt/sapphire and Pt/Ti/SiO2/Si substrates with pulsed laser deposition using the same growth conditions, respectively. Au was sputtered as the top electrode. The microscopic structure of the thin film varies by changing the underlying substrate. Thin films on Pt/sapphire are not resistively switchable due to the formation of Schottky contacts at both the top and the bottom interface. However, thin films on Pt/Ti/SiO2/Si exhibit an obvious resistive switching behavior under forward bias. The conduction mechanisms in BiFeO3 thin films on Pt/sapphire and Pt/Ti/SiO2/Si substrates are discussed to understand the different resistive switching behaviors.",1209.5868v1 2012-10-22,"Thickness-dependent structural, magnetic and transport properties of epitaxial Co2FeAl Heusler alloy thin films","We report on a systematic study of the structural, magnetic properties and the anomalous Hall effect, in the Heusler alloy Co2FeAl (CFA) epitaxial films on MgO(001), as a function of film thickness. It was found that the epitaxial CFA films show a highly ordered B2 structure with an in-plane uniaxial magnetic anisotropy. An analysis of the electrical transport properties reveals that the lattice and magnon scattering contributions to the longitudinal resistivity. Independent on the thickness of films, the anomalous Hall resistivity of CFA films is found to be dominated by skew scattering only. Moreover, the anomalous Hall resistivity shows weakly temperature dependent behavior, and its absolute value increases as the thickness decreases. We attribute this temperature insensitivity in the anomalous Hall resistivity to the weak temperature dependent of tunneling spin-polarization in the CFA films, while the thickness dependence behavior is likely due to the increasing significance of interface or free surface electronic states.",1210.5807v1 2012-12-06,Barkhausen-type noise in the resistance of antiferromagnetic Cr thin films,"We present an experimental study of the changes generated on the electrical resistance $R(T)$ of epitaxial Cr thin films by the transformation of quantized spin density wave domains as the temperature is changed. A characteristic resistance noise appears only within the same temperature region where a cooling-warming cycle in $R(T)$ displays hysteretic behavior. We propose an analysis based on an analogy with the Barkhausen noise seen in ferromagnets. There fluctuations in the magnetization $M(H)$ occur when the magnetic field $H$ is swept. By mapping $M \rightarrow \Psi_0$ and $H \rightarrow T$, where $\Psi_0$ corresponds to the order parameter of the spin density wave, we generalize the Preisach model in terms of a random distribution of {\it resistive hysterons} to explain our results. These hysterons are related to distributions of quantized spin density wave domains with different sizes, local energies and number of nodes.",1212.1411v1 2012-12-10,YCr6Ge6 as a Candidate Compound for a Kagome Metal,"We show that YCr6Ge6, comprising a kagome lattice made up of Cr atoms, is a plausible candidate compound for a kagome metal that is expected to exhibit anomalous phenomena such as flat-band ferromagnetism. Resistivity, magnetization, and heat capacity are measured on single crystals of YCr6Ge6, and band structure calculations are performed to investigate the electronic structure. Curie-Weiss-like behavior in magnetic susceptibility, T2 dependence in resistivity, and a Sommerfeld coefficient doubly enhanced from a calculated value indicate a moderately strong electron correlation. Interestingly, the in-plane resistivity is twice as large as the interplane resistivity, which is contrary to the simple expectation from the layered structure. Band structure calculations demonstrate that there are partially flat bands slightly below the Fermi level near the {\Gamma} point, which is ascribed to Cr 3d3z2-r2 bands and may govern the properties of this compound.",1212.1976v1 2013-03-26,Quantum corrections to conductivity in Si doped ZnO thin films,"Si doped ZnO thin films with Si concentrations ranging from 0.4 to 10 % have been grown by sequential pulsed laser deposition on sapphire substrates. The resistivity of the films first decreased from ~ 6.6x10-3 to 4.7x10-4 ohm-cm as the Si concentration was increased from ~ 0.4 to 2% and then it increased with further increase in Si concentration. The electron concentrations in the films were in the range from 3x1019 to 4x1020 cm-3 showing their degenerate nature. However, temperature dependent resistivity measurements in the range from 300 to 4.2 K revealed negative temperature coefficient of resistivity (TCR) for the 0.4, 6 and 10% Si doped ZnO films in the entire measurement temperature range. The 0.6, 0.9 and 2% Si doped films showed a transition from negative to positive TCR with increasing temperature. The negative magnetoresistance found in the films at low temperatures and 0.5 T magnetic field pointed to weak localization as the dominant contributor towards negative TCR. A quantitative fit of the temperature dependent resistivity data for all the films could be obtained by considering the quantum correction to conductivity arising due to disorder induced weak localization effect.",1303.6443v2 2013-08-29,Percolation model for a selective response of the resistance of composite semiconducting np-systems towards reducing gases,"It is shown that a two-component percolation model can explain an experimentally observed behavior, namely that a network built up by a mixture of sintered nanocrystalline semiconducting n- and p-grains can exhibit selective behavior, i.e. respond with a resistance increase when exposed to a reducing gas A and with a resistance decrease in response to another reducing gas B. To this end, a simple model is developed based on realistic assumptions about the reactions on the grain surfaces. The resistance is calculated by random walk simulations with nn-, pp- and np-bonds between the grains and the results are found in very good agreement with the experiments. Contrary to former assumptions, the np-bonds are crucial to obtain this accordance.",1308.6442v2 2013-11-08,Low-Contact-Resistance Graphene Devices with Nickel-Etched-Graphene Contacts,"The performance of graphene-based transistors is often limited by the large electrical resistance across the metal-graphene contact. We report an approach to achieve ultra-low resistance metal contacts to graphene transistors. Through a process of metal-catalyzed etching in hydrogen, multiple nano-sized pits with zigzag edges are created in the graphene that form strong chemical bonds with deposited nickel metallization for source-drain contacts without the need for further annealing. This facile contact treatment prior to electrode metallization results in contact resistance as low as 100 ohm-um in single-layer graphene field-effect transistors, and 11 ohm-um in bilayer graphene transistors. The treatment is compatible with complementary metal-oxide-semiconductor fabrication processes, and holds great promise to meet the contact performance required for the integration of graphene in future integrated circuits.",1311.1944v2 2014-06-14,Negative magnetoresistance dynamics in expanded graphite under hydrostatic pressure up to 1.8 GPa,"Basal plane resistivity of expanded graphite was studied under simultaneous influence of hydrostatic pressure up to 1.8 GPa and magnetic field 0.8 T in the 77-300 K temperature region. Magnetic field induces negative magnetoresistance in the sample within all temperature and pressure range studied. A change in resistivity of the sample under maximum pressure reaches 80%. Significant change in resistivity dependence on temperature under the pressure of 0.6 GPa suggests for ordering transition in the sample studied. Negative magnetoresistance in the graphite reaches about 15% at 0.6 GPa. Magnetic field acts in the same way as pressure and potentiates the transition formation and further magnetoresistance dynamics. The effects observed are mostly of elastic character according to resistivity of the unloaded sample.",1406.3770v1 2014-06-23,Control of Thermoelectric Properties of ZnO using Electric Double Layer,"We have successfully controlled thermoelectric properties of ZnO by changing carrier concentration using an electric double layer transistor (EDLT) which is a feld effect transistor gated by electrolyte solution. The resistivity and the thermopower decreased abruptly by applying gate voltage larger than a threshold voltage ( 2V), indicating the increase of carrier concentration on the ZnO surface. The temperature dependence of resistivity became metallic, which is characterized by weak temperature dependence of the resistivity, when gate voltage exceeded 2V. Corresponding to the resistivity, the temperature dependence of thermopower changed remarkably. The thickness of the induced metallic layer was estimated to be about 10nm from the critical carrier concentration of metal-insulator transition, and the power factor was calculated to ~8*10-5Wm-1K2. Although the power factor is not as large as bulk ZnO ceramics of optimum doping condition, EDLT is considered to be a useful way to optimize thermoelectric properties by tuning carrier concentration.",1406.5850v1 2014-09-28,Universal Ratio of Intrinsic Resistivities of Spin Helix in B20 (Fe-Co)Si Magnets,"The B20 magnets with the Dzyaloshinskii-Moriya (D-M) interaction exhibit spin helix and Skyrmion spin textures unattainable in traditional Heisenberg ferromagnets. We have determined the intrinsic resistivity of the spin helix, which is a macroscopic Bloch domain wall, in B20 (Fe-Co)Si magnets. We found a universal resistance ratio of gamma = 1.35 with current parallel and perpendicular to the helix, independent of composition and temperature. This gamma value is much smaller than 3, the well-known minimum value for domain wall resistivity in traditional ferromagnets, due to the significant spin-orbit coupling in the B20 magnets.",1409.7869v1 2014-11-13,Graphene-Passivated Nickel as an Oxidation-Resistant Electrode for Spintronics,"We report on graphene-passivated ferromagnetic electrodes (GPFE) for spin devices. GPFE are shown to act as spin-polarized oxidation-resistant electrodes. The direct coating of nickel with few layer graphene through a readily scalable chemical vapour deposition (CVD) process allows the preservation of an unoxidized nickel surface upon air exposure. Fabrication and measurement of complete reference tunneling spin valve structures demonstrates that the GPFE is maintained as a spin polarizer and also that the presence of the graphene coating leads to a specific sign reversal of the magneto-resistance. Hence, this work highlights a novel oxidation-resistant spin source which further unlocks low cost wet chemistry processes for spintronics devices.",1411.3476v1 2014-11-22,"Crystal growth, resistivity and Hall effect of the delafossite metal PtCoO$_2$","We report single crystal growth of the delafossite oxide PtCoO$_2$, and basic transport measurements on single crystals etched to well-defined geometries using focused ion beam techniques. The room temperature resistivity is 2.1 $\mu\Omega$ cm, and the Hall coefficient is consistent with the existence of one free electron per Pt. Although the residual resistivity ratio is greater than fifty, a slight upturn of resistivity is seen below 15 K. The angle dependence of the in-plane magnetoresistance is also reported.",1411.6162v2 2015-03-02,High-Q operation of SRF cavities: The potential impact of thermocurrents on the RF surface resistance,"For many new accelerator applications, superconducting radio frequency (SRF) systems are the enabling technology. In particular for CW applications, much effort is being expended to minimize the power dissipation (surface resistance) of niobium cavities. Starting in 2009, we suggested a means of reducing the residual resistance by performing a thermal cycle [1], a procedure of warming up a cavity after initial cooldown to about 20K and cooling it down again. In subsequent studies [2], this technique was used to manipulate the residual resistance by more than a factor of 2. It was postulated that thermocurrents during cooldown generate additional trapped magnetic flux that impacts the cavity quality factor. Here, we present a more extensive study that includes measurements of two additional passband modes and that confirms the effect. In this paper, we also discuss simulations that support the claim. While the layout of the cavity LHe tank system is cylindrically symmetric, we show that the temperature dependence of the material parameters results in a non-symmetric current distribution. Hence a significant amount of magnetic flux can be generated at the RF surface.",1503.00601v2 2015-05-28,Effect of the interface resistance in non-local Hanle measurements,"We use lateral spin valves with varying interface resistance to measure non-local Hanle effect in order to extract the spin-diffusion length of the non-magnetic channel. A general expression that describes spin injection and transport, taking into account the influence of the interface resistance, is used to fit our results. Whereas the fitted spin-diffusion length value is in agreement with the one obtained from standard non-local measurements in the case of a finite interface resistance, in the case of transparent contacts a clear disagreement is observed. The use of a corrected expression, recently proposed to account for the anisotropy of the spin absorption at the ferromagnetic electrodes, still yields a deviation of the fitted spin-diffusion length which increases for shorter channel distances. This deviation shows how sensitive the non-local Hanle fittings are, evidencing the complexity of obtaining spin transport information from such type of measurements.",1505.07592v1 2016-01-25,Lower limits of line resistance in nanocrystalline Back End of Line Cu interconnects,"The strong non-linear increase in Cu interconnect line resistance with a decrease in linewidth presents a significant obstacle to their continued downscaling. In this letter we use first principles density functional theory based electronic structure of Cu interconnects to find the lower limits of their line resistance for metal linewidths corresponding to future technology nodes. We find that even in the absence of scattering due to grain boundaries, edge roughness or interfaces, quantum confinement causes a severe reduction in current carrying capacity of Cu. We discuss the causes of transport orientation dependent anisotropy of quantum confinement in Cu. We also find that when the simplest scattering mechanism in the grain boundary scattering dominated limit is added to otherwise coherent electronic transmission in monocrystalline nanowires, the lower limits of line resistance are significantly higher than projected roadmap requirements in the International Technology Roadmap for Semiconductors.",1601.06675v2 2016-05-12,NdCeCuO - NdCeO boundary and resistive switchings in mesoscopic structures on base of epitaxial NdCeCuO films,"Reverse and stable bipolar resistive switching effect was observed in planar NdCeCuO - NdCeO - Ag heterostructures. It was shown that the current voltage charactereriscs of the BRSE observed has a diode character. Simulations were used to consider the influence of the nonuniform distribution of an electric field at the interface of a heterojunction on the effect of bipolar resistive switching in investigated structures. The inhomogeneous distribution of the electric field near the contact edge creates regions of higher electric field strength which, in turn, stimulates motion and redistribution of defects, changes of the resistive properties of the whole structure and formation of a percolation channel.",1605.03913v1 2016-08-25,Resistive Switching in Aqueous Nanopores by Shock Electrodeposition,"Solid-state programmable metallization cells have attracted considerable attention as memristive elements for Redox-based Resistive Random Access Memory (ReRAM) for low-power and low-voltage applications. In principle, liquid-state metallization cells could offer the same advantages for aqueous systems, such as biomedical lab-on-a-chip devices, but robust resistive switching has not yet been achieved in liquid electrolytes, where electrodeposition is notoriously unstable to the formation of fractal dendrites. Here, the recently discovered physics of shock electrodeposition are harnessed to stabilize aqueous copper growth in polycarbonate nanopores, whose surfaces are modified with charged polymers. Stable bipolar resistive switching is demonstrated for 500 cycles with <10s retention times, prior to any optimization of the geometry or materials.",1608.07007v1 2017-02-17,An alternative to the spin-coupled interface resistance for describing heat generation,"Using a macroscopic approach, we studied theoretically the heat generation in a typical spin valve with nonmagnetic spacer layer of finite thickness. Our analysis shows that the spin-dependent heat generation cannot be interpreted as the Joule heating of the spin-coupled interface resistance except for some special segments. Moreover, the spin-coupled interface resistance can be negative in certain situation, and thus its ""Joule heating"" should be understood instead as the work done by the extra field in the ferromagnetic layers and at the spin-selective interfaces. Effective resistances are proposed as alternatives so that the spin-dependent heat generation can still be expressed in a form resembling Joule's law.",1702.05283v1 2017-09-27,Kapitza thermal resistance across individual grain boundaries in graphene,"We study heat transport across individual grain boundaries in suspended monolayer graphene using extensive classical molecular dynamics (MD) simulations. We construct bicrystalline graphene samples containing grain boundaries with symmetric tilt angles using the two-dimensional phase field crystal method and then relax the samples with MD. The corresponding Kapitza resistances are then computed using nonequilibrium MD simulations. We find that the Kapitza resistance depends strongly on the tilt angle and shows a clear correlation with the average density of defects in a given grain boundary, but is not strongly correlated with the grain boundary line tension. We also show that quantum effects are significant in quantitative determination of the Kapitza resistance by applying the mode-by-mode quantum correction to the classical MD data. The corrected data are in good agreement with quantum mechanical Landauer-B\""utticker calculations.",1709.09529v1 2017-12-08,A Novel Effect of Electron Spin Resonance on Electrical Resistivity,"We extend the well known phenomenon of magnetoresistance (extra resistivity of materials in transverse magnetic field) to a new and unexplored regime where in addition to a transverse magnetic field, a transverse AC field of resonant frequency is also applied. In a magnetic field, electron spin levels are Zeeman split. In a resonant AC field, we uncover a new channel of momentum relaxation in which electrons in upper Zeeman level can deexcite to lower Zeeman level by generating spin fluctuation excitation in the lattice (similar to what happens in Electron Spin Resonance (ESR) spectroscopy). An additional resistivity due to this novel mechanism is predicted in which momentum randomization of Zeeman split electrons happen via bosonic excitations (spin fluctuations). An order of magnitude of this additional resistivity is calculated. The whole work is based upon an extension of Einstein's derivation of equilibrium Planckian formula to near equilibrium systems.",1712.03062v1 2017-12-11,Finite Size Effects in Highly Scaled Ruthenium Interconnects,"Ru has been considered a candidate to replace Cu-based interconnects in VLSI circuits. Here, a methodology is proposed to predict the resistivity of (Ru) interconnects. First, the dependence of the Ru thin film resistivity on the film thickness is modeled by the semiclassical Mayadas-Shatzkes (MS) approach. The fitting parameters thus obtained are then used as input in a modified MS model for nanowires to calculate wire resistivities. Predicted experimental resistivities agreed within about 10%. The results further indicate that grain boundary scattering was the dominant scattering mechanism in scaled Ru interconnects.",1712.03859v2 2017-12-23,A micromechanics-based analytical solution for the effective thermal conductivity of composites with orthotropic matrices and interfacial thermal resistance,"We obtained an analytical solution for the effective thermal conductivity of composites composed of orthotropic matrices and spherical inhomogeneities with interfacial thermal resistance using a micromechanics-based homogenization. We derived the closed form of a modified Eshelby tensor as a function of the interfacial thermal resistance. We then predicted the heat flux of a single inhomogeneity in the infinite media based on the modified Eshelby tensor, which was validated against the numerical results obtained from the finite element analysis. Based on the modified Eshelby tensor and the localization tensor accounting for the interfacial resistance, we derived an analytical expression for the effective thermal conductivity tensor for the composites by a mean-field approach called the Mori-Tanaka method. Our analytical prediction matched very well with the effective thermal conductivity obtained from finite element analysis with up to 10% inhomogeneity volume fraction.",1712.08715v2 2019-09-06,Strong suppression of the resistivity near the transition to superconductivity in narrow micro-bridges in external magnetic fields,"We have investigated a series of superconducting bridges based on homogeneous amorphous WSi and MoSi films, with bridge widths w ranging from 2 um to 1000 um and film thicknesses d ~ 4-6 nm and 100 nm. Upon decreasing the bridge widths below the respective Pearl lengths, we observe in all cases distinct changes in the characteristics of the resistive transitions to superconductivity. For each of the films, the resistivity curves R(B,T) separate at a well-defined and field-dependent temperature T*(B) with decreasing the temperature, resulting in a dramatic suppression of the resistivity and a sharpening of the transitions with decreasing bridge width w. The associated excess conductivity in all the bridges scales as 1/w, which may suggest the presence of a highly conducting region that is dominating the electric transport in narrow bridges. We argue that this effect can only be observed in materials with sufficiently weak vortex pinning.",1909.02915v2 2019-09-13,Tunable resistivity exponents in the metallic phase of epitaxial nickelates,"We report a detailed analysis of the electrical resistivity exponent of thin films of NdNiO3 as a function of epitaxial strain. Strain-free thin-films show a linear dependence of the resistivity vs temperature, consistent with a classical Fermi gas ruled by electron-phonon interactions. In addition, the apparent temperature exponent, n, can be tuned with the epitaxial strain between n= 1 and n= 3. We discuss the critical role played by quenched random disorder in the value of n. Our work shows that the assignment of Fermi/Non-Fermi liquid behaviour based on experimentally obtained resistivity exponents requires an in-depth analysis of the degree of disorder in the material.",1909.06256v1 2014-08-08,Effects of Lifshitz Transition on Charge Transport in Magnetic Phases of Fe-Based Superconductors,"The unusual temperature dependence of the resistivity and its in-plane anisotropy observed in the Fe-based superconducting materials, particularly Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$, has been a longstanding puzzle. Here we consider the effect of impurity scattering on the temperature dependence of the average resistivity within a simple two-band model of a dirty spin density wave metal. The sharp drop in resistivity below the N\'eel temperature $T_N$ in the parent compound can only be understood in terms of a Lifshitz transition following Fermi surface reconstruction upon magnetic ordering. We show that the observed resistivity anisotropy in this phase, arising from nematic defect structures, is affected by the Lifshitz transition as well.",1408.1933v3 2019-07-01,A perspective on effective medium models of thermal conductivity in (ultra)nanocrystalline diamond films,"Thermal conductivity of nanocrystalline and ultra-nanocrystalline films is analyzed with effective medium theory (EMT) models. The existing EMT models use the spherical inclusion approximation. Although this approximation works quite well it is inconsistent, mostly with respect to the maximal packing of 74{\%}, which may be unrealistic for polycrystalline films. To check the consistency of these models we devise an EMT model with arbitrarily shaped inclusions. We pick the EMT model with cubic inclusions and we compare its results with the results of the EMT model with spherical inclusions. It is found a very good agreement between both calculations. This agreement is explained by general geometrical arguments. We further employ these models to analyze thermal conductivity of nanocrystalline and ultra-nanocrystalline diamond films. It is noticed that the effective conductivity is strongly affected not only by the boundary Kapitza resistance but also by intra-grain scattering for grain sizes below 100 nm. Generally, both intra-grain conductivity and Kapitza resistance increase with grain size. However, the effect of Kapitza resistance increase is negligible due to the geometrical factor accompanying Kapitza resistance contribution to the effective conductivity.",1907.00753v1 2016-03-02,Giant Frictional Drag in Double Bilayer Graphene Heterostructures,"We study the frictional drag between carriers in two bilayer graphene flakes separated by a 2 $-$ 5 nm thick hexagonal boron nitride dielectric. At temperatures ($T$) lower than $\sim$ 10 K, we observe a large anomalous negative drag emerging predominantly near the drag layer charge neutrality. The anomalous drag resistivity increases dramatically with reducing {\it T}, and becomes comparable to the layer resistivity at the lowest {\it T} = 1.5 K. At low $T$ the drag resistivity exhibits a breakdown of layer reciprocity. A comparison of the drag resistivity and the drag layer Peltier coefficient suggests a thermoelectric origin of this anomalous drag.",1603.00757v1 2017-04-05,Stateful characterization of resistive switching TiO2 with electron beam induced currents,"Metal oxide resistive switches are increasingly important as possible artificial synapses in next generation neuromorphic networks. Nevertheless, there is still no codified set of tools for studying properties of the devices. To this end, we demonstrate electron beam induced current measurements as a powerful method to monitor the development of local resistive switching in TiO2 based devices. By comparing beam-energy dependent electron beam induced currents with Monte Carlo simulations of the energy absorption in different device layers, it is possible to deconstruct the origins of filament image formation and relate this to both morphological changes and the state of the switch. By clarifying the contrast mechanisms in electron beam induced current microscopy it is possible to gain new insights into the scaling of the resistive switching phenomenon and observe the formation of a current leakage region around the switching filament. Additionally, analysis of symmetric device structures reveals propagating polarization domains.",1704.01475v2 2017-08-31,Antiferromagnetic anisotropy determination by spin Hall magnetoresistance,"An electric method for measuring magnetic anisotropy in antiferromagnetic insulators (AFIs) is proposed. When a metallic film with strong spin-orbit interactions, e.g., platinum (Pt), is deposited on an AFI, its resistance should be affected by the direction of the AFI N eel vector due to the spin Hall magnetoresistance (SMR). Accordingly, the direction of the AFI N eel vector, which is affected by both the external magnetic field and the magnetic anisotropy, is reflected in resistance of Pt. The magnetic field angle dependence of the resistance of Pt on AFI is calculated by consider- ing the SMR, which indicates that the antiferromagnetic anisotropy can be obtained experimentally by monitoring the Pt resistance in strong magnetic fields. Calculations are performed for realistic systems such as Pt/Cr2O3, Pt/NiO, and Pt/CoO.",1708.09564v1 2019-08-12,Graphene-based spinmechatronic valve,"Interlayer twist between van der Waals graphene crystals led to the discovery of superconducting and insulating states near the magic angle. In this work, we exploit this mechanical degree of freedom by twisting the graphene middle layer in a trilayer graphene spacer between two metallic lead (Magnetic and nonmagnetic). A large difference in conductance is found depending on the angle of twist between the middle layer graphene and the ones at the interface this difference, called twisting resistance, reach more than 1000% in the non-magnetic Cu case. For the magnetic Ni case, the magneto-resistance decreases and the difference in conductance between twisted and not twisted depends strongly on the relative magnetization configuration. For the parallel configuration, the twisting resistance is about -40%, while for the anti-parallel configuration it can reach up to 130%. Furthermore, we show that the twisting resistance can be enhanced by inserting a thin Cu layer at the interface of Ni/graphene where it reaches a value of 200% and 1600% for parallel and antiparallel configurations, respectively. These finding could pave the way toward the integration of 2D materials on novel spinmechatronics based devices.",1908.04076v1 2019-08-15,Observation of Highly Nonlinear Resistive Switching of Al2O3/TiO2-x Memristors at Cryogenic Temperature (1.5 K),"In this work, we investigate the behavior of Al2O3/TiO2-x cross-point memristors in cryogenic environment. We report successful resistive switching of memristor devices from 300 K down to 1.5 K. The I-V curves exhibit negative differential resistance effects between 130 and 1.5 K, attributed to a metal-insulator transition (MIT) of the Ti4O7 conductive filament. The resulting highly nonlinear behavior is associated to a maximum ION/IOFF ratio of 84 at 1.5 K, paving the way to selector-free cryogenic passive crossbars. Finally, temperature-dependant thermal activation energies related to the conductance at low bias (20 mV) are extracted for memristors in low resistance state, suggesting hopping-type conduction mechanisms.",1908.05545v4 2018-07-28,Anomalous Hall Effect and Spin Fluctuations in Ionic Liquid Gated SrCoO$_3$ Thin Films,"The recent realization of epitaxial SrCoO$_3$ thin films has triggered a renewed interest in their electronic, magnetic, and ionic properties. Here we uncover several unusual magneto-transport properties of this compound, suggesting that it hosts persistent spin fluctuation down to low temperatures. We achieve the metallic SrCoO$_3$ with record-low resistivity from insulating SrCoO$_{2.5}$ by the ionic liquid gating. We find a linear relationship between the anomalous Hall resistivity and the longitudinal resistivity, which cannot be accounted for by the conventional mechanisms. We theoretically propose that the impurity induced chiral spin fluctuation gives rise to such a dependence. The existence of spin fluctuation manifests itself as negatively enhanced magneto-resistance of SrCoO$_3$ when the temperature approaches zero. Our study brings further insight into the unique spin state of SrCoO$_3$ and unveils a novel skew scattering mechanism for the anomalous Hall effect.",1807.10877v1 2019-01-14,Phonon and electronic structures and resistance of layered electride Ca2N: DFT calculations,"The phonon and electronic properties, the Eliashberg function and the temperature dependence of resistance of electride Ca2N are investigated by the DFT-LDA plane-wave method. The phonon dispersion, the partial phonon density of states and the atomic eigenvectors of zero-center phonons are studied. The electronic band dispersion and partial density of states conclude that Ca2N is a metal and the Ca 3p, 4s and N 2p orbitals are hybridized. For the analysis of an electron - phonon interaction (EPI) and its contribution to resistance the Eliashberg function was calculated and a temperature dependence of resistance caused EPI was found. The present results are in good agreement with experiment data.",1901.04594v1 2020-05-22,VoteAgain: A scalable coercion-resistant voting system,"The strongest threat model for voting systems considers coercion resistance: protection against coercers that force voters to modify their votes, or to abstain. Existing remote voting systems either do not provide this property; require an expensive tallying phase; or burden users with the need to store cryptographic key material and with the responsibility to deceive their coercers. We propose VoteAgain, a scalable voting scheme that relies on the revoting paradigm to provide coercion resistance. VoteAgain uses a novel deterministic ballot padding mechanism to ensure that coercers cannot see whether a vote has been replaced. This mechanism ensures tallies take quasilinear time, making VoteAgain the first revoting scheme that can handle elections with millions of voters. We prove that VoteAgain provides ballot privacy, coercion resistance, and verifiability; and we demonstrate its scalability using a prototype implementation of all cryptographic primitives.",2005.11189v3 2020-06-06,Radiative Resistance at The Nano-scale: Thermal Barrier,"In present article the radiative thermal current and radiative resistance are introduced and investigated in a system of parallel slabs. The system is placed in an environment with a constant temperature and subjected to a constant temperature gradient, which causes a radiative energy flux through the system. We have calculated the steady-state temperatures profile of the system, assuming that the material and thickness of the middle slab could be different from the other slabs. We propose the exact formulation for calculating the thermal current and thermal resistances in both linear and nonlinear regimes. According to our results, the middle slab acts as a thermal barrier and depending on the width of this barrier, an extreme thermal isolation is achievable. Simulation results indicate that the thermal resistance of the barrier is an increasing function of the thickness for near-field separation distances but it is virtually insensitive to the barrier width in far field regime. The long range character of the radiative heat transfer, which occurs in system with identical slabs is also discussed.",2006.03842v4 2020-08-16,Strange metal behavior of the Hall angle in twisted bilayer graphene,"Twisted bilayer graphene (TBG) with interlayer twist angles near the magic angle $\approx 1.08^{\circ}$ hosts flat bands and exhibits correlated states including Mott-like insulators, superconductivity and magnetism. Here we report combined temperature-dependent transport measurements of the longitudinal and Hall resistivities in close to magic-angle TBG. While the observed longitudinal resistivity follows linear temperature $T$ dependence consistent with previous reports, the Hall resistance shows an anomalous $T$ dependence with the cotangent of the Hall angle cot $\Theta{_H} \propto T^2$. Boltzmann theory for quasiparticle transport predicts that both the resistivity and cot $\Theta{_H}$ should have the same $T$ dependence, contradicting the observed behavior. This failure of quasiparticle-based theories is reminiscent of other correlated strange metals such as cuprates.",2008.06907v1 2020-08-23,Negative resistance state in superconducting NbSe$_2$ induced by surface acoustic waves,"We report a negative resistance, namely, a voltage drop along the opposite direction of a current flow, in the superconducting gap of NbSe$_2$ thin films under the irradiation of surface acoustic waves (SAWs). The amplitude of the negative resistance becomes larger by increasing the SAW power and decreasing temperature. As one possible scenario, we propose that soliton-antisoliton pairs in the charge density wave of NbSe$_2$ modulated by the SAW serve as a time-dependent capacitance in the superconducting state, leading to the dc negative resistance. The present experimental result would provide a previously unexplored way to examine nonequilibrium manipulation of the superconductivity.",2008.09948v1 2020-11-17,Effect of Substrate Roughness on Oxidation Resistance of an Aluminized Ni-Base Superalloy,"In the present work, it is shown that the surface preparation method used on two Ni-based superalloys prior to aluminizing chemical vapor deposition (CVD) is one of the most important factors determining the oxidation resistance of aluminized Ni-based superalloys. It was found that grit blasting the substrate surface negatively affects the oxidation resistance of the aluminized coatings. For grit blasted and aluminized IN 625, a thicker outer NiAl coating was formed compared to that of IN 738. In contrast, no effect on NiAl coating thickness was found for grit blasted and aluminized IN 738. However, a thicker interdiffusion zone (IDZ) was observed. It was shown that the systems with grit-blasted surfaces reveal worse oxidation resistance during thermal shock tests, namely, a higher mass loss was observed for both grit blasted and aluminized alloys, as compared to ground and aluminized alloys. A possible reason for this effect of remaining alumina particles originating from surface grit blasting on the diffusion processes and stress distribution at the coating/substrate is proposed.",2011.08921v1 2021-04-23,Microstructure and wear resistance of Fe-Cr-C-Mo-V-Ti-N hardfacing layers,"In this paper, to improve wear resistance of components such as screws under severe friction-wear, Fe-Cr-C-Mo-V-Ti-N hardfacing coatings were further developed. The hardfacing coatings were acquired by shielded manual arc welding (SMAW) method. The ferroalloys added into the coating flux of the hardfaced electrode were jointly nitrided. The microstructure of the coatings was carried out using X-ray diffraction(XRD), optical microscope(OM), field emission scanning electron microscope (FESEM) and energy dispersive Xray spectrometry (EDS). In addition, FactSage 7.0 software was employed to calculate the equilibrium phase diagram of the hardfacings. The wear resistance was performed on a pin-on-disc machine. The Fe-Cr-C- Mo-V-Ti-N hardfacings exhibited higher wear resistance than cladding layer without nitrides.",2104.11402v1 2021-05-27,Systematic manipulation of the surface conductivity of SmB$_6$,"We show that the resistivity plateau of SmB$_6$ at low temperature, typically taken as a hallmark of its conducting surface state, can systematically be influenced by different surface treatments. We investigate the effect of inflicting an increasing number of hand-made scratches and microscopically defined focused ion beam-cut trenches on the surfaces of flux-grown Sm$_{1-x}$Gd$_x$B$_6$ with $x =$ 0, 0.0002. Both treatments increase the resistance of the low-temperature plateau, whereas the bulk resistance at higher temperature largely remains unaffected. Notably, the temperature at which the resistance deviates from the thermally activated behavior decreases with cumulative surface damage. These features are more pronounced for the focused ion beam treated samples, with the difference likely being related to the absence of microscopic defects like subsurface cracks. Therefore, our method presents a systematic way of controlling the surface conductance.",2105.13057v1 2021-06-23,A new symmetry-based extraction method of Schottky diode parameters from resistance-compensated I-V characteristics,"We present a novel resistance-compensated I-V method to extract the series resistance, ideality factor, barrier height and built-in potential of a metal-semiconductor diode. We show that a reduced equation arises from a unique but hitherto unreported symmetry in the Schottky equation when it is written as an ordinary differential equation. In spite of the intense mathematical justification, we show how this new equation is directly applicable to an empirical data set through a simple algorithm. We test the method on a new Al/p-Si/Bi$_2$Se$_3$/Al Schottky diode and compare it with the Cheung-Cheung method on the same data. The series resistance was found to change exponentially with applied bias with a rate constant that depends on the incident illumination. The barrier height decreased with bias but was independent of the incident illumination. The trends in the results of the method agree strongly with the literature and may yield more accurate diode parameters compared to other electrical methods.",2106.12324v1 2021-08-19,Influence of charged walls and defects on DC resistivity and dielectric relaxation in Cu-Cl boracite,"Charged domain walls form spontaneously in Cu-Cl boracite on cooling through the phase transition. These walls exhibit changed conductivity compared to the bulk and motion consistent with the existence of negative capacitance. Here, we present the dielectric permittivity and DC resistivity of bulk Cu-Cl boracite as a function of temperature (-140 {\deg}C to 150 {\deg}C) and frequency (1 mHz to 10 MHz). The thermal behaviour of the two observed dielectric relaxations and the DC resistivity is discussed. We propose that the relaxations can be explained by the existence of point defects, most likely local complexes created by a change of valence of Cu and accompanying oxygen vacancies. In addition, the sudden change in resistivity seen at the phase transition suggests that conductive domain walls contribute significantly to the conductivity in the ferroelectric phase.",2108.08582v2 2022-01-10,Designs for programmable quantum resistance standards based on epitaxial graphene p-n junctions,"We report the fabrication and measurement of top gated epitaxial graphene p-n junctions where exfoliated hexagonal boron nitride (h-BN) is used as the gate dielectric. The four-terminal longitudinal resistance across a single junction is well quantized at the von Klitzing constant R_K with a relative uncertainty of 10-7. After the exploration of numerous parameter spaces, we summarize the conditions upon which these devices could function as potential resistance standards. Furthermore, we offer designs of programmable electrical resistance standards over six orders of magnitude by using external gating.",2201.03621v1 2022-04-26,"Nonreciprocal electrical transport in multiferroic semiconductor (Ge,Mn)Te","We have investigated the nonreciprocal electrical transport, that is a nonlinear resistance effect depending on the current direction, in multiferroic Rashba semiconductor (Ge,Mn)Te. Due to coexistence of ferromagnetic and ferroelectric orders, (Ge,Mn)Te provides a unique platform for exploring the nonreciprocal electrical transport in a bulk form. (Ge,Mn)Te thin films shows a large nonreciprocal resistance compared to GeTe, the nonmagnetic counterpart with the same crystal structure. The magnetic-field-angle dependence of the nonreciprocal resistance is maximized when magnetic field is orthogonal to both current and electric polarization, in accord with the symmetry argument. From the analysis of temperature and magnetic field dependence, we deduce that inelastic scatterings of electrons mediated by magnons dominantly contribute to the observed nonreciprocal response. Furthermore, the nonreciprocal resistance is significantly enhanced by lowering hole density. The Fermi level dependence is attributed to the deformation of the Rashba band in which the spin-momentum locked single Fermi surface appears by exchange field from the in-plane magnetization. The present study provides a key insight to the mechanisms of novel transport phenomena caused by the interplay of ferroelectric and ferromagnetic orders in a semiconductor.",2204.12427v1 2022-08-17,Transport properties of dipole skyrmions in amorphous FeGd multilayers,"The transport response of dipole skyrmions in amorphous centrosymmetric Fe/Gd multilayer is investigated by temperature and field-dependent resistivity measurements collected in three current and magnetic field configurations. It is shown that a dipole skyrmion lattice phase may form at certain temperatures leading to a unique signature of the polar longitudinal resistivity. This signature differs from the conventional field-varying parabolic response associated with stripe phases, which transition to a disordered skyrmion phase under applied fields. Transport measurements under different field history protocols reveal that the anomaly in the polar longitudinal resistivity appears under specific field history reversal processes. Our experimental results are reproduced using micromagnetic simulations that show the anomaly in the polar longitudinal resistivity is related to a domain wall reconfiguration that occurs as the domain morphology transitions from disordered stripes to a skyrmion lattice under applied perpendicular fields.",2208.08487v1 2023-01-18,Synthesizing $2h/e^2$ resistance plateau at the first Landau level confined in a quantum point contact,"A comprehensive understanding of quantum Hall edge transmission, especially the hole-conjugate of a Laughlin state such as a $2/3$ state, is critical for advancing fundamental quantum Hall physics and enhancing the design of quantum Hall edge interferometry. In this study, we report a robust intermediate $2h/e^2$ resistance quantization in a quantum point contact (QPC) when the bulk is set at the fractional filling $2/3$ quantum Hall state. Our results suggest the occurrence of two equilibration processes. First, the co-propagating $1/3$ edges moving along a soft QPC arm confining potential fully equilibrate and act as a single $2/3$ edge mode. Second, the $2/3$ edge mode is further equilibrated with an integer $1$ edge mode formed in the QPC. The complete mixing between them results in a diagonal resistance value quantized at $2h/e^2$. Similar processes occur for a bulk filling $5/3$, leading to an intermediate $(2/3)h/e^2$ resistance quantization.",2301.07488v2 2024-02-28,Impact of etches on thin-film single-crystal niobium resonators,"A single crystal niobium thin film was grown using molecular beam epitaxy on a c-plane sapphire wafer. Several samples were fabricated into dc resistivity test devices and coplanar waveguide resonator chips using the same microfabrication procedures and solvent cleans. The samples were then subject to different acid cleaning treatments using different combinations of piranha, hydrofluoric acid, and buffered oxide etch solutions. The different samples expressed changes in dc resistivity in the normal and superconducting states such that the low temperature resistivities changed by more than 100\%, and the residual resistivity ratio dropped by a factor of 2. The internal quality factor of coplanar waveguide resonators measured near 5~GHz also showed significant variation at single photon powers ranging from 1.4$\times 10^6$ to less than 60$\times 10^3$. These changes correlate with the formation of surface crystallites that appear to be hydrocarbons. All observations are consistent with hydrogen diffusing into the niobium film at levels below the saturation threshold that is needed to observe niobium hydrides.",2402.18051v1 2024-05-02,Optimization of reactively sputtered Mn3GaN films based on resistivity measurements,"Mn-based nitrides with antiperovskite structures have several properties that can be utilised for antiferromagnetic spintronics. Their magnetic properties depend on the structural quality, composition and doping of the cubic antiperovskite structure. Such nitride thin films are usually produced by reactive physical vapour deposition, where the deposition rate of N can only be controlled by the N2 gas flow. We show that the tuning of the N content can be optimised using low temperature resistivity measurements, which serve as an indicator of the degree of structural disorder. Several Mn3GaNx films were prepared by reactive magnetron sputtering under different N2 gas flows. Under optimised conditions, we obtain films that exhibit a metal-like temperature dependence, a vanishing logarithmic increase in resistivity towards zero, the highest resistivity ratio and a lattice contraction of 0.4 % along the growth direction when heated above that of the N\'eel temperature in agreement with the bulk samples.",2405.01203v1 2004-02-04,A simple estimate of the electron hopping energy in the Bechgaard salts,"Starting from a previously derived theoretical expression for the electrical conductivity of the Bechgaard salts,and experimental data on the resistivity of these materials,it is shown how a valueof the electron hopping energy can be determined.Values obtained in this way are in agreement with estimates made by more complicated methods.",0402127v1 2019-09-12,Gallium Nitride FET Model,"We have presented an analytical physics-based compact model of GaN power FET, which can accurately describe the I-V characteristics in all operation modes. The model considers the source-drain resistance, different interface trap densities and self-heating effects.",1909.05702v1 2019-09-18,A current-voltage characteristic of photoresistance. A plane case,"The formation of photo-electron current in the volume of semi-conductor material is investigated in this article. A plane case when a material is uniformly illuminated by light is considered. The current-voltage characteristic of a photo resistance is obtained in analytical form.",1909.09135v1 2019-10-04,The Test of Topological Property of YbB6,"Topological insulator is a recently discovered class of material with topologically protected surface state. YbB6 is predicted to be moderately correlated Z2 topological insulator similar to SmB6. Here, I experimentally test the resistance property of bulk YbB6 to verify its topological property. By changing the thickness of YbB6, I found out that although the data curves did not completely conform to the theory of topology, the experimental observation to the overall trend showed a similar topological phenomenon.",1910.02056v1 2020-01-25,Exfoliation of Two-Dimensional Nanosheets of Metal Diborides,"The metal diborides are a class of ceramic materials with crystal structures consisting of hexagonal sheets of boron atoms alternating with planes of metal atoms held together with mixed character ionic/covalent bonds. Many of the metal diborides are ultrahigh temperature ceramics like HfB$_2$, TaB$_2$, and ZrB$_2$, which have melting points above 3000$^\circ$C, high mechanical hardness and strength at high temperatures, and high chemical resistance, while MgB$_2$ is a superconductor with a transition temperature of 39 K. Here we demonstrate that this diverse family of non-van der Waals materials can be processed into stable dispersions of two-dimensional (2D) nanosheets using ultrasonication-assisted exfoliation. We generate 2D nanosheets of the metal diborides AlB$_2$, CrB$_2$, HfB$_2$, MgB$_2$, NbB$_2$, TaB$_2$, TiB$_2$, and ZrB$_2$, and use electron and scanning probe microscopies to characterize their structures, morphologies, and compositions. The exfoliated layers span up to micrometers in lateral dimension and reach thicknesses down to 2-3 nm, while retaining their hexagonal atomic structure and chemical composition. We exploit the convenient solution-phase dispersions of exfoliated CrB$_2$ nanosheets to incorporate them directly into polymer composites. In contrast to the hard and brittle bulk CrB$_2$, we find that CrB$_2$ nanocomposites remain very flexible and simultaneously provide increases in the elastic modulus and the ultimate tensile strength of the polymer. The successful liquid-phase production of 2D metal diborides enables their processing using scalable low-temperature solution-phase methods, extending their use to previously unexplored applications, and reveals a new family of non-van der Waals materials that can be efficiently exfoliated into 2D forms.",2001.09237v1 2005-10-07,"Collective Spin and Charge Excitations in (Sr,La)_{14-x}Ca_xCu_{24}O_{41} Quantum Spin Ladders","We study magnetic and electronic properties of two-leg ladder materials. We observed a two-magnon (2M) resonance which we analyze in terms of symmetry, relaxation and resonance properties. Our findings were contrasted to 2M Raman measurements in other magnetic crystals. This comparison made us suggest that the spin-spin correlations in a self-doped two leg ladder may have a modulated component besides the exponential decay characteristic of a spin liquid ground state. We found that the 2M intensity resonates at the Mott gap energy. Interplane Sr substitution for Ca introduces strong disorder leading to inhomogeneous broadening of the 2M resonance. The doped holes in the spin liquid ground state further dilute the magnetic correlations, suppressing the spectral weight of this excitation. At high Ca concentrations are superconducting under pressure and hole pairing was proposed to be a robust feature of doped ladders. The measured dielectric response in the microwave region, the low energy Raman data, the non-linear transport properties along with soft x-ray scattering allowed us to conclude that the ground state for a wide range of Ca concentrations (x < 12) is characterized by charge density wave correlations. This state seems to be driven not by phonons but by Coulomb forces and many-body effects. We highlighted the similarity in the finite frequency Raman response as opposed to the very different behavior of the DC resistivity between undoped and doped ladders. We found that at high Ca concentrations the carrier relaxation is characterized by the same large activation energy (~2000 K) as in the self-doped compound. This observation prompted us to suggest an unconventional metallic transport driven by collective electronic response.",0510193v1 2009-02-13,Nanoscale Electronic Inhomogeneity in In2Se3 Nanoribbons Revealed by Microwave Impedance Microscopy,"Driven by interactions due to the charge, spin, orbital, and lattice degrees of freedom, nanoscale inhomogeneity has emerged as a new theme for materials with novel properties near multiphase boundaries. As vividly demonstrated in complex metal oxides and chalcogenides, these microscopic phases are of great scientific and technological importance for research in high-temperature superconductors, colossal magnetoresistance effect, phase-change memories, and domain switching operations. Direct imaging on dielectric properties of these local phases, however, presents a big challenge for existing scanning probe techniques. Here, we report the observation of electronic inhomogeneity in indium selenide (In2Se3) nanoribbons by near-field scanning microwave impedance microscopy. Multiple phases with local resistivity spanning six orders of magnitude are identified as the coexistence of superlattice, simple hexagonal lattice and amorphous structures with 100nm inhomogeneous length scale, consistent with high-resolution transmission electron microscope studies. The atomic-force-microscope-compatible microwave probe is able to perform quantitative sub-surface electronic study in a noninvasive manner. Finally, the phase change memory function in In2Se3 nanoribbon devices can be locally recorded with big signal of opposite signs.",0902.2255v1 2009-10-01,Template engineering of Co-doped BaFe2As2 single-crystal thin films,"Understanding new superconductors requires high-quality epitaxial thin films to explore intrinsic electromagnetic properties, control grain boundaries and strain effects, and evaluate device applications. So far superconducting properties of ferropnictide thin films appear compromised by imperfect epitaxial growth and poor connectivity of the superconducting phase. Here we report novel template engineering using single-crystal intermediate layers of (001) SrTiO3 and BaTiO3 grown on various perovskite substrates that enables genuine epitaxial films of Co-doped BaFe2As2 with high transition temperature (zero resistivity Tc of 21.5K), small transition widths (delta Tc = 1.3K), superior Jc of 4.5 MA/cm2 (4.2K, self field) and strong c-axis flux pinning. Implementing SrTiO3 or BaTiO3 templates to match the alkaline earth layer in the Ba-122 with the alkaline earth-oxygen layer in the templates opens new avenues for epitaxial growth of ferropnictides on multi-functional single crystal substrates. Beyond superconductors, it provides a framework for growing heteroepitaxial intermetallic compounds on various substrates by matching interfacial layers between templates and thin film overlayers.",0910.0268v1 2009-11-19,Large transport critical currents of powder-in-tube Sr0.6K0.4Fe2As2/Ag superconducting wires and tapes,"We report significant transport critical currents firstly achieved in Sr0.6K0.4Fe2As2 wires and tapes with a Tc = 34 K, which were fabricated through an in-situ powder-in-tube process. Silver was used as a chemical addition as well as a sheath material. Transport measurements were performed by a standard four-probe resistive method. All the wire and tape samples have shown transport properties. Critical current density Jc was enhanced upon silver addition, and at 4.2 K, a best Jc of ~1200 A/cm^2 (Ic = 9 A) was achieved for 20 % silver added tapes, which is the highest in iron-based wires and tapes so far. The Jc is almost field independent between 1 T and 10 T, exhibiting a strong vortex pinning. Such a high transport critical current density is attributed to the absence of reaction layer between the silver sheath and superconducting core, as well as an improved connectivity between grains. We also identify a weak-link behavior from the creep drop of Jc at low fields and a hysteretic phenomenon. Finally, we found that compared to Fe, Ta and Nb tubes, Ag was the best sheath material for the fabrication of high-performance 122 type pnictide wires and tapes.",0911.3701v1 2010-10-05,Hierarchical formation of bulgeless galaxies: Why outflows have low angular momentum,"Using high resolution, fully cosmological smoothed particle hydro-dynamical simulations of dwarf galaxies in a Lambda cold dark matter Universe, we show how baryons attain a final angular momentum distribution which allows pure disc galaxies to form. Blowing out substantial amounts of gas through supernovae and stellar winds, which is well supported observationally, is a key ingredient in forming bulgeless discs. We outline why galactic outflows preferentially remove low angular momentum material, and show that this is a natural result when structure forms in a cold dark matter cosmology. The driving factors are a) the mean angular momentum of accreted material increases with time, b) lower potentials at early times, c) the existence of an extended reservoir of high angular momentum gas which is not within star forming regions, meaning that only gas from the inner region (low angular momentum gas) is expelled and d) the tendency for outflows to follow the path of least resistance which is perpendicular to the disc. We also show that outflows are enhanced during mergers, thus expelling much of the gas which has lost its angular momentum during these events, and preventing the formation of ""classical"", merger driven bulges in low mass systems. Stars formed prior to such mergers form a diffuse, extended stellar halo component.",1010.1004v3 2014-02-13,On the spheroidized carbide dissolution and elemental partitioning in a high carbon bearing steel 100Cr6,"We report on the characterization of high carbon bearing steel 100Cr6 using electron microscopy and atom probe tomography in combination with multi-component diffusion simulations (DICTRA). Scanning electron micrographs show that around 14 vol.% spheroidized carbides are formed during soft annealing and only 3 vol.% remain after dissolution into the austenitic matrix by austenitization at 1123 K (850 {\deg}C) for 300 s. The spheroidized particles are identified as (Fe, Cr)3C by transmission electron microscopy. Atom probe analyses reveal the redistribution and partitioning behaviors of elements, i.e. C, Si, Mn, Cr, Fe in both, the spheroidized carbides and the bainitic matrix in the sample isothermally heat-treated at 773 K (500 {\deg}C) after austenitization. A homogeneous distribution of C and gradual gradient of Cr was detected within the spheroidized carbides. Due to its limited diffusivity in (Fe, Cr)3C, Cr exhibits a maximum concentration at the surface of spheroidized carbides (16 at.%) and decreases gradually from surface towards the core down to a level of about 2 at.%. The atom probe results also indicate that the partially dissolved spheroidized carbides during austenitization may serve as nucleation sites for intermediate temperature cementite within bainite, which results in a relatively softer surface and harder core in spheroidized particles. This microstructure may contribute to the good wear resistance and fatigue properties",1402.3315v1 2014-05-23,Proof-of-principle of a new geometry for sampling calorimetry using inorganic scintillator plates,"A novel geometry for a sampling calorimeter employing inorganic scintillators as an active medium is presented. To overcome the mechanical challenges of construction, an innovative light collection geometry has been pioneered, that minimises the complexity of construction. First test results are presented, demonstrating a successful signal extraction. The geometry consists of a sampling calorimeter with passive absorber layers interleaved with layers of an active medium made of inorganic scintillating crystals. Wavelength-shifting (WLS) fibres run along the four long, chamfered edges of the stack, transporting the light to photodetectors at the rear. To maximise the amount of scintillation light reaching the WLS fibres, the scintillator chamfers are depolished. It is shown herein that this concept is working for cerium fluoride (CeF$_3$) as a scintillator. Coupled to it, several different types of materials have been tested as WLS medium. In particular, materials that might be sufficiently resistant to the High-Luminosity Large Hadron Collider radiation environment, such as cerium-doped Lutetium-Yttrium Orthosilicate (LYSO) and cerium-doped quartz, are compared to conventional plastic WLS fibres. Finally, an outlook is presented on the possible optimisation of the different components, and the construction and commissioning of a full calorimeter cell prototype is presented.",1405.6202v1 2015-02-10,Emergence of the minority hole with high mobility on the electrical transport in the Fe-pnictides Ba(Fe$_{1-x}$Mn$_x$As)$_2$,"In Fe pnictide (Pn) superconducting materials, neither Mn- nor Cr- doping to the Fe site induces superconductivity, even though hole carriers are generated. This is in strong contrast with the superconductivity appearing when holes are introduced by alkali metal substitution on the insulating blocking layers. We investigate in detail the effects of Mn doping on magneto-transport properties in Ba(Fe$_{1-x}$Mn$_x$As)$_2$ for elucidating the intrinsic reason. The negative Hall coefficient for $x$ = 0 estimated in the low magnetic field ($B$) regime gradually increases as $x$ increases, and its sign changes to a positive one at $x$ = 0.020. Hall resistivities as well as simultaneous interpretation using the magnetoconductivity tensor including both longitudinal and transverse transport components clarify that minority holes with high mobility are generated by the Mn doping via spin density wave (SDW) transition at low temperatures, while original majority electrons and holes residing in the parabolic-like Fermi surfaces (FSs) of the semimetallic Ba(FeAs)$_2$ are negligibly affected. Present results indicate that the mechanism of hole doping in Ba(Fe$_{1-x}$Mn$_x$As)$_2$ is greatly different from that of the other superconducting FePns family.",1502.02845v3 2015-08-16,Surface States Engineering of Metal/MoS2 Contacts Using Sulfur Treatment for Reduced Contact Resistance and Variability,"Variability and lack of control in the nature of contacts between metal/MoS2 interface is a major bottleneck in the realisation of high-performance devices based on layered materials for several applications. In this letter, we report on the reduction in Schottky barrier height at metal/MoS2 interface by engineering the surface states through sulphur treatment. Electrical characteristics for back-gated MoS2 field effect transistor structures were investigated for two high work-function metal contacts Ni and Pd. Contacts on MoS2 treated with sulphur exhibited significant improvements in Ohmic nature with concomitant reduction in variability compared to those on untreated MoS2 films leading to a 2x increase in extracted mobility. X-ray Photoelectron Spectroscopy (XPS) measurements, Raman Spectroscopy and comparison of threshold voltages indicated absence of additional doping or structural changes due to sulphur treatment. The Schottky barrier heights were extracted from temperature-dependent transfer characteristics based on the thermionic current model. A reduction in barrier height of 80 and 135 meV extracted for Ni/MoS2 and Pd/MoS2 contacts respectively is hence attributed to the increase in surface states (or stronger Fermi level pinning) due to sulphur treatment. The corresponding charge neutrality levels at metal/MoS2 interface, were extracted to be 0.16 eV (0.17 eV) below the conduction band before (after) Sulphur treatment. This first report of surface states engineering in MoS2 leading to superior contacts is expected to significantly benefit the entire class of devices based on layered 2D materials.",1508.03795v2 2016-06-28,Method for Transferring High-Mobility CVD-Grown Graphene with Perfluoropolymers,"The transfer of graphene grown by chemical vapor deposition (CVD) using amorphous polymers represents a widely implemented method for graphene-based electronic device fabrication. However, the most commonly used polymer, poly(methyl methacrylate) (PMMA), leaves a residue on the graphene that limits the mobility. Here we report a method for graphene transfer and patterning that employs a perfluoropolymer---Hyflon---as a transfer handle and to protect graphene against contamination from photoresists or other polymers. CVD-grown graphene transferred this way onto LaAlO$_3$/SrTiO$_3$ heterostructures is atomically clean, with high mobility (~30,000 cm$^2$V$^{-1}$s$^{-1}$) near the Dirac point at 2 K and clear, quantized Hall and magneto-resistance. Local control of the LaAlO$_3$/SrTiO$_3$ interfacial metal-insulator transition---through the graphene---is preserved with this transfer method. The use of perfluoropolymers such as Hyflon with CVD-grown graphene and other 2D materials can readily be implemented with other polymers or photoresists.",1606.08802v1 2016-10-31,High Electric Field Carrier Transport and Power Dissipation in Multilayer Black Phosphorus Field Effect Transistor with Dielectric Engineering,"This study addresses high electric field transport in multilayer black phosphorus (BP) field effect transistors (FETs) with self-heating and thermal spreading by dielectric engineering. Interestingly, we found that multilayer BP device on a SiO2 substrate exhibited a maximum current density of 3.3 x 10E10 A/m2 at an electric field of 5.58 MV/m, several times higher than multilayer MoS2. Our breakdown thermometry analysis revealed that self-heating was impeded along BP-dielectric interface, resulting in a thermal plateau inside the channel and eventual Joule breakdown. Using a size-dependent electro-thermal transport model, we extracted an interfacial thermal conductance of 1-10 MW/m2 K for the BP-dielectric interfaces. By using hBN as a dielectric material for BP instead of thermally resistive SiO2 (about 1.4 W/m K), we observed a 3 fold increase in breakdown power density and a relatively higher electric field endurance together with efficient and homogenous thermal spreading because hBN had superior structural and thermal compatibility with BP. We further confirmed our results based on micro-Raman spectroscopy and atomic force microscopy, and observed that BP devices on hBN exhibited centrally localized hotspots with a breakdown temperature of 600K, while the BP device on SiO2 exhibited a hotspot in the vicinity of the electrode at 520K.",1610.09951v1 2017-02-02,High-Pressure Synthesis and Characterization of $β$-GeSe - A Semiconductor with Six-Rings in an Uncommon Boat Conformation,"Two-dimensional materials have significant potential for the development of new devices. Here we report the electronic and structural properties of $\beta$-GeSe, a previously unreported polymorph of GeSe, with a unique crystal structure that displays strong two-dimensional structural features. $\beta$-GeSe is made at high pressure and temperature and is stable under ambient conditions. We compare it to its structural and electronic relatives $\alpha$-GeSe and black phosphorus. The $\beta$ form of GeSe displays a boat conformation for its Ge-Se six-ring, while the previously known $\alpha$ form, and black phosphorus, display the more common chair conformation for their six-rings. Electronic structure calculations indicate that $\beta$-GeSe is a semiconductor, with an approximate bulk band gap of $\Delta~\approx$ 0.5 eV, and, in its monolayer form, $\Delta~\approx$ 0.9 eV. These values fall between those of $\alpha$-GeSe and black phosphorus, making $\beta$-GeSe a promising candidate for future applications. The resistivity of our $\beta$-GeSe crystals measured in-plane is on the order of $\rho \approx$ 1 $\Omega$cm, while being essentially temperature independent.",1702.00715v1 2017-09-21,Effect of nanostructure on thermoelectric properties of La$_{0.7}$Sr$_{0.3}$MnO$_{3}$ in 300-600 K range,"In oxide materials, nanostructuring effect has been found very promising approach for the enhancement of \textit{figure-of-merit}, \textit{ZT}. In the present work, we have synthesized La$_{0.7}$Sr$_{0.3}$MnO$_{3}$ (LSMO) compound using sol-gel method and samples of crystallite size of 34, 41, and 49 nm were obtained by giving different heat treatment. Seebeck coefficient ($\alpha$), electrical resistivity ($\rho$), and thermal conductivity ($\kappa$) measurements were carried out in 300-600 K temperature range. The systematic change in the values of $\alpha$ from $\sim$ -19 $\mu$V/K to $\sim$ -24 $\mu$V/K and drastic reduction in the values of $\kappa$ from $\sim$0.88 W/mK to $\sim$0.23 W/mK are observed as crystallite size is reduced from 49 nm to 34 nm at $\sim$600 K. Also, fall in the values of $\rho$ in the paramagnetic (PM) insulator phase (400-600 K) are effectively responsible for the increasing trend in the values of \textit{ZT} at high temperature. For the crystallite size of 41 nm, value of \textit{ZT} at 600 K was found to be $\sim$0.017, which can be further increased up to $\sim$0.045 around 650 K temperature. The predicted value of \textit{ZT} suggests that LSMO can be suitable oxide material for thermoelectric applications at high temperature.",1709.07205v2 2017-12-17,Short range order in the quantum XXZ honeycomb lattice material BaCo$_2$(PO$_4$)$_2$,"We present observations of highly frustrated quasi two-dimensional (2D) magnetic correlations in the honeycomb lattice layers of the S$_{eff}$ = 1/2 compound $\gamma$-BaCo$_2$(PO$_4$)$_2$ ($\gamma$-BCPO). Specific heat shows a broad peak comprised of two weak kink features at $T_{N1} \sim$ 6 K and $T_{N2} \sim$ 3.5 K, the relative weights of which can be modified by sample annealing. Neutron powder diffraction measurements reveal short range quasi-2D order that is established below $T_{N1}$ and $T_{N2}$, at which two separate, incompatible, short range magnetic orders onset: commensurate antiferromagnetic correlations with correlation length $\xi_c = 60\pm2$ \AA \ ($T_{N1}$) and in quasi-2D helical domains with $\xi_h = 350 \pm 11$ \AA \ ($T_{N2}$). The ac magnetic susceptibility response lacks frequency dependence, ruling out spin freezing. Inelastic neutron scattering data on $\gamma$-BCPO is compared with linear spin wave theory, and two separate parameter regions of the XXZ $J_1$-$J_2$-$J_3$ model with ferromagnetic nearest-neighbor exchange $J_1$ are favored, both near regions of high classical degeneracy. High energy coherent excitations ($\sim 10$ meV) persist up to at least 40 K, suggesting strong in-plane correlations persist above $T_N$. These data show that $\gamma$-BCPO is a rare highly frustrated, quasi-2D S$_{eff}$ = 1/2 honeycomb lattice material which resists long range magnetic order and spin freezing.",1712.06208v2 2018-02-22,Touch Sensors with Overlapping Signals: Concept Investigation on Planar Sensors with Resistive or Optical Transduction,"Traditional methods for achieving high localization accuracy on tactile sensors usually involve a matrix of miniaturized individual sensors distributed on the area of interest. This approach usually comes at a price of increased complexity in fabrication and circuitry, and can be hard to adapt to non-planar geometries. We propose a method where sensing terminals are embedded in a volume of soft material. Mechanical strain in this material results in a measurable signal between any two given terminals. By having multiple terminals and pairing them against each other in all possible combinations, we obtain a rich signal set using few wires. We mine this data to learn the mapping between the signals we extract and the contact parameters of interest. Our approach is general enough that it can be applied with different transduction methods, and achieves high accuracy in identifying indentation location and depth. Moreover, this method lends itself to simple fabrication techniques and makes no assumption about the underlying geometry, potentially simplifying future integration in robot hands.",1802.08209v2 2018-11-27,Unifying Description of Competing Orders in Two Dimensional Quantum Magnets,"Quantum magnets provide the simplest example of strongly interacting quantum matter, yet they continue to resist a comprehensive understanding above one spatial dimension (1D). In 1D, a key ingredient to progress is Luttinger liquid theory which provides a unified description. Here we explore a promising analogous framework in two dimensions, the Dirac spin liquid (DSL), which can be constructed on several different lattices. The DSL is a version of Quantum Electrodynamics ( QED$_3$) with four flavors of Dirac fermions coupled to photons. Importantly, its excitations also include magnetic monopoles that drive confinement. By calculating the complete action of symmetries on monopoles on the square, honeycomb, triangular and kagom\`e lattices, we answer previously open key questions. We find that the stability of the DSL is enhanced on the triangular and kagom\`e lattices as compared to the bipartite (square and honeycomb) lattices. We obtain the universal signatures of the DSL on the triangular and kagom\`e lattices, including those that result from monopole excitations, which serve as a guide to numerics and to experiments on existing materials. Interestingly, the familiar 120 degree magnetic orders on these lattices can be obtained from monopole proliferation. Even when unstable, the Dirac spin liquid unifies multiple ordered states which could help organize the plethora of phases observed in strongly correlated two-dimensional materials.",1811.11186v2 2017-03-18,The Effect of Temperature on Cu-K-In-Se Thin Films,"Films of Cu-K-In-Se were co-evaporated at varied K/(K+Cu) compositions and substrate temperatures (with constant (K+Cu)/In ~ 0.85). Increased Na composition on the substrate's surface and decreased growth temperature were both found to favor Cu1-xKxInSe2 (CKIS) alloy formation, relative to mixed-phase CuInSe2 + KInSe2 formation. Structures from X-ray diffraction (XRD), band gaps, resistivities, minority carrier lifetimes and carrier concentrations from time-resolved photoluminescence were in agreement with previous reports, where low K/(K+Cu) composition films exhibited properties promising for photovoltaic (PV) absorbers. Films grown at 400-500 C were then annealed to 600 C under Se, which caused K loss by evaporation in proportion to initial K/(K+Cu) composition. Similar to growth temperature, annealing drove CKIS alloy consumption and CuInSe2 + KInSe2 production, as evidenced by high temperature XRD. Annealing also decomposed KInSe2 and formed K2In12Se19. At high temperature the KInSe2 crystal lattice gradually contracted as temperature and time increased, as well as just time. Evaporative loss of K during annealing could accompany the generation of vacancies on K lattice sites, and may explain the KInSe2 lattice contraction. This knowledge of Cu-K-In-Se material chemistry may be used to predict and control minor phase impurities in Cu(In,Ga)(Se,S)2 PV absorbers-where impurities below typical detection limits may have played a role in recent world record PV efficiencies that utilized KF post-deposition treatments.",1703.06366v1 2019-02-26,Bonding and oxidation protection of Ti${_2}$AlC and Cr${_2}$AlC for a Ni-based Superalloy,"Alumina forming, oxidation and thermal shock resistant MAX phases are of a high interest for high temperature applications. Herein we report, on bonding and resulting interactions between a Ni-based superalloy, NSA, and two alumina forming MAX phases. The diffusion couples Cr${_2}$AlC/Inconel-718/Ti${_2}$AlC were assembled and heated to 1000 or 1100{\deg}C in a vacuum hot press under loads corresponding to stresses of either 2 MPa or 20 MPa. The resulting interfaces were examined using X-ray diffraction, scanning electron microscopy and energy-dispersive X-ray spectroscopy. Good bonding between Cr${_2}$AlC and NSA was achieved after hot pressing at 1000{\deg}C and a contact pressure of only 2 MPa; in the case of Ti${_2}$AlC a higher temperature (1100{\deg}C) and pressure (20 MPa) were needed. In both cases, a diffusion bond was realized with no evidence of interfacial damage or cracking after cooling to room temperature. Twenty thermal cycles from room temperature to 1000{\deg}C showed that Ti${_2}$AlC is a poor oxidation barrier for Inconel-718. However, in the case of Cr${_2}$AlC no cracks, delamination nor surface degradation were observed, suggesting that this material could be used to protect Inconel-718 from oxidation.",1902.10001v2 2020-04-22,Deformation of micrometer and mm-sized Fe2.4wt.%Si single- and bi-crystals with a high angle grain boundary at room temperature,"Plasticity in body-centred cubic (BCC) metals, including dislocation interactions at grain boundaries, is much less understood than in face-centred cubic (FCC) metals. At low temperatures additional resistance to dislocation motion due to the Peierls barrier becomes important, which increases the complexity of plasticity. Iron-silicon steel is an interesting, model BCC material since the evolution of the dislocation structure in specifically-oriented grains and at particular grain boundaries have far-reaching effects not only on the deformation behaviour but also on the magnetic properties, which are important in its final application as electrical steel. In this study, two different orientations of micropillars (1, 2, 4 microns in diameter) and macropillars (2500 microns) and their corresponding bi crystals are analysed after compression experiments with respect to the effect of size on strength and dislocation structures. Using different experimental methods, such as slip trace analysis, plane tilt analysis and cross-sectional EBSD, we show that direct slip transmission occurs, and different slip systems are active in the bi-crystals compared to their single-crystal counterparts. However, in spite of direct transmission and a very high transmission factor, dislocation pile-up at the grain boundary is also observed at early stages of deformation. Moreover, an effect of size scaling with the pillar size in single crystals and the grain size in bi-crystals is found, which is consistent with investigations elsewhere in FCC metals.",2004.10598v2 2022-02-01,Strong Edge Stress in Molecularly Thin Organic$-$Inorganic Hybrid Ruddlesden$-$Popper Perovskites and Modulations of Their Edge Electronic Properties,"Organic$-$inorganic hybrid Ruddlesden$-$Popper perovskites (HRPPs) have gained much attention for optoelectronic applications due to their high moisture resistance, good processibility under ambient conditions, and long functional lifetimes. Recent success in isolating molecularly thin hybrid perovskite nanosheets and their intriguing edge phenomena have raised the need for understanding the role of edges and the properties that dictate their fundamental behaviours. In this work, we perform a prototypical study on the edge effects in ultrathin hybrid perovskites by considering monolayer (BA)$_2$PbI$_4$ as a representative system. Based on first-principles simulations of nanoribbon models, we show that in addition to significant distortions of the octahedra network at the edges, strong edge stresses are also present in the material. Structural instabilities that arise from the edge stress could drive the relaxation process and dominate the morphological response of edges in practice. A clear downward shift of the bands at the narrower ribbons, as indicative of the edge effect, facilitates the separation of photo-excited carriers (electrons move towards the edge and holes move towards the interior part of the nanosheet). Moreover, the desorption energy of the organic molecule can also be much lower at the free edges, making it easier for functionalization and/or substitution events to take place. The findings reported in this work elucidate the underlying mechanisms responsible for edge states in HRPPs and will be important in guiding the rational design and development of high-performance layer$-$edge devices.",2202.00296v1 2016-03-11,Quantum Critical Behavior in a Concentrated Ternary Solid Solution,"Quantum critical behavior has been associated with some of the most exotic emergent states of matter including high-temperature superconductivity. Much of the research into quantum critical point (QCP) physics has been hampered by the lack of model systems simple enough to be analyzed by theory. Here, we show that the concentrated solid solution fcc alloys, including the so-called high-entropy alloys, are ideal model systems to study the effects of chemical disorder on emergent properties near a quantum critical region. The face centered cubic (fcc) alloy NiCoCrx with x near 1 is found to be close to the Cr concentration where the ferromagnetic transition temperature, Tc, goes to 0. Near this composition these alloys exhibit a resistivity linear in temperature to 2 K, a linear magnetoresistance, an excess -TlnT contribution to the low temperature heat capacity and excess low temperature entropy. All of the low temperature electrical, magnetic and thermodynamic properties of the alloys with compositions near x near 1 are not typical of a Fermi liquid and suggest strong magnetic fluctuations associated with a quantum critical region. The limit of extreme chemical disorder in these simple fcc materials thus provides a novel and unique platform to study quantum critical behavior in a highly tunable system.",1603.03781v1 2019-03-09,Dry transfer method for suspended graphene on lift-off-resist: simple ballistic devices with Fabry-Pérot interference,"We demonstrate a fabrication scheme for clean suspended structures using chemical-vapor-deposition-grown graphene and a dry transfer method on lift-off-resist-coated substrates to facilitate suspended graphene nanoelectronic devices for technology applications. It encompasses the demands for scalable fabrication as well as for ultra-fast response due to weak coupling to environment. The fabricated devices exhibited initially a weak field-effect response with substantial positive ($p$) doping which transformed into weak negative ($n$) doping upon current annealing at the temperature of 4 Kelvin. With increased annealing current, $n$-doping gradually decreased while the Dirac peak position approached zero in gate voltage. An ultra-low residual charge density of $9\times10^8 \mathrm{ \ cm^{-2}}$ and a mobility of $1.9 \times 10^5 \mathrm{\ cm^2/Vs}$ were observed. Our samples display clear Fabry-P\'{e}rot (FP) conductance oscillation which indicates ballistic electron transport. The spacing of the FP oscillations are found to depend on the charge density in a manner that agrees with theoretical modeling based on Klein tunneling of Dirac particles. The ultra-low residual charge, the FP oscillations with density dependent period, and the high mobility prove excellent quality of our suspended graphene devices. Owing to its simplicity, scalability and robustness, this fabrication scheme enhances possibilities for production of suspended, high-quality, two-dimensional-material structures for novel electronic applications.",1903.03780v1 2019-12-11,Quantum oscillations and electronic structures in large Chern number semimetal RhSn,"We report the magnetoresistance, Hall effect, de Haas-van Alphen (dHvA) oscillations and the electronic structures of single crystal RhSn, which is a typical material of CoSi family holding a large Chern number. The large unsaturated magnetoresistance is observed with B//[001]. The Hall resistivity curve indicates that RhSn is a multi-band system with high mobility. Evident quantum oscillations have been observed, from which the light effective masses are extracted. Ten fundamental frequencies are extracted after the fast Fourier transform analysis of the dHvA oscillations with B//[001] configuration. The two low frequencies F$_1$ and F$_2$ do not change obviously and the two high frequencies F$_9$ and F$_{10}$ evolve into four when B rotates from B//[001] to B//[110], which is consistent with the band structure in the first-principles calculations with spin-orbit coupling (SOC). The extracted Berry phases of the relative pockets show a good agreement with the Chern number $\pm4$ (with SOC) in the first-principles calculations. Above all, our studies indicate that RhSn is an ideal platform to study the unconventional chiral fermions and the surface states.",1912.05148v1 2019-12-11,Bulk and Two-dimensional Silver and Copper Monohalides: A Unique Class of Materials with Modest Ionicity/Covalency and Ferroelasticity/Multiferroicity,"Silver and copper monohalides can be viewed as a class of compounds in the neutral zone between predominantly covalent and ionic compounds, thereby exhibiting neither strong ionicity nor strong covalency. We show ab initio calculation evidence that silver and copper monohalides entail relatively low transition barriers between the non-polar rock-salt phase and the polar zinc-blende phase, due largely to their unique chemical nature of modest iconicity or covalency. Notably, the low transition barriers endow both monohalides with novel mechanical and electronic properties, i.e., coupled ferroelasticity and ferroelectricity with large polarizations and relatively low switching barriers at ambient conditions. Several halides even possess very similar lattice constants and structures as the prevailing semiconductors such as silicon, thereby enabling epitaxial growth on silicon. Moreover, based on extensive structural search, we find that the most stable two-dimensional (2D) polymorphs of the monolayer halides are close or even greater in energy than their bulk counterparts, a feature not usually seen in the family of rock-salt or zinc-blende semiconductors. The low transition barrier between zinc-blende phase and 2D phase is predicted. Moreover, several 2D monolayer halides also exhibit multiferroicity with coupled ferroelasticity or ferroelectricity, thereby rendering their potential applications as high-density integrated memories for efficient data reading and writing. Their surfaces, covered by halides, also provide oxidation resistance and give low cleave energy from layered structure, suggesting high likelihood of experimental synthesis of these 2D polymorphs.",1912.05172v1 2015-04-14,Carrier Transport at the Metal-MoS2 Interface,"This study illustrates the nature of electronic transport and its transition from one mechanism to another between a metal electrode and MoS2 channel interface in a field effect transistor (FET) device. Interestingly, measurements of the contact resistance (Rc) as a function of temperature indicate a transition in the carrier transport across the energy barrier from a thermionic emission at a high temperature to tunneling at a low temperature. Furthermore, at a low temperature, the nature of the tunneling behavior is ascertained by the current-voltage dependency that helps us feature direct tunneling at a low bias and Fowler-Nordheim tunneling at a high bias for a Pd-MoS2 contact due to the effective barrier shape modulation by biasing. In contrast, only direct tunneling is observed for a Cr-MoS2 contact over the entire applied bias range. In addition, simple analytical calculations were carried out to extract Rc at the gating range, and the results are consistent with the experimental data. Our results describe the transition in carrier transport mechanisms across a metal-MoS2 interface, and this information provides guidance for the design of future flexible, transparent electronic devices based on 2-dimensional materials.",1504.03466v1 2018-12-28,Nanoscale Self-Healing Mechanisms in Shape Memory Ceramics,"Shape memory (SM) ceramics, such as yttria-stabilized tetragonal zirconia (YSTZ), are a unique family of SM materials that offer unique properties including ultra-high operating temperature, and high resistance to chemical corrosion and oxidation. However, formation of defects is usually observed in SM ceramics during manufacturing and/or by mechanical deformation. To fully take advantage of the SM properties of these ceramics, it is necessary to fully understand the nano-structural evolution of defects under external stimuli. In this study, defect closure behaviors in YSTZ nanopillars are investigated by atomistic simulations. Two characteristic orientations of [011-] and [001] are selected to represent the dominant deformation mechanisms of phase transformation and dislocation migration, respectively. With the presence of crack and void, the strength and yield strain of nanopillars are noted to decrease significantly, especially for [011-]-oriented YSTZ nanopillars. Volume expansion associated with the tetragonal to monoclinic phase transformation is observed to promote healing of crack and void. Atom stress analyses reveal stress concentrations along the newly formed monoclinic phase bands. A critical crack width is identified, less than which the crack can be fully closed in compression. Size effect study reveals that an increase in nanopillar size has a positive effect on crack self-healing behavior. For [001]-oriented YSTZ nanopillars, dislocation migration leads to formations of an amorphous phase, which also assist the crack and void closure process. The revealed crack/void healing mechanisms may provide a path for mitigating internal defects that influences the mechanical properties and deformation mechanisms of SM ceramics.",1812.11136v1 2019-06-24,Melting of vortex lattice in magnetic superconductor $\mathrm{Rb}\mathrm{Eu}\mathrm{Fe}_{4}\mathrm{As}_{4}$,"The iron-based superconductors are characterized by strong fluctuations due to high transition temperatures and small coherence lengths. We investigate fluctuation behavior in the magnetic iron-pnictide superconductor $\mathrm{Rb}\mathrm{Eu}\mathrm{Fe}_{4}\mathrm{As}_{4}$ by calorimetry and transport. We find that the broadening of the specific-heat transition in magnetic fields is very well described by the lowest-Landau-level scaling. We report calorimetric and transport observations for vortex-lattice melting, which is seen as a sharp drop of the resistivity and a step of the specific heat at the magnetic-field-dependent temperature. The melting line in the temperature/magnetic-field plane lies noticeably below the upper-critical-field line and its location is in quantitative agreement with theoretical predictions without fitting parameters. Finally, we compare the melting behavior of $\mathrm{Rb}\mathrm{Eu}\mathrm{Fe}_{4}\mathrm{As}_{4}$ with other superconducting materials showing that thermal fluctuations of vortices are not as prevalent as in the high-temperature superconducting cuprates, yet they still noticeably influence the properties of the vortex matter.",1906.10236v2 2020-01-23,Magnetic-field-induced robust zero Hall plateau state in MnBi$_2$Te$_4$ Chern insulator,"The intrinsic antiferromagnetic topological insulator MnBi2Te4 provides an ideal platform for exploring exotic topological quantum phenomena. Recently, the Chern insulator and axion insulator phases have been realized in few-layer MnBi2Te4 devices at low magnetic field regime. However, the fate of MnBi2Te4 in high magnetic field has never been explored in experiment. In this work, we report transport studies of exfoliated MnBi2Te4 flakes in pulsed magnetic fields up to 61.5 T. In the high-field limit, the Chern insulator phase with Chern number C = -1 evolves into a robust zero Hall resistance plateau state. Nonlocal transport measurements and theoretical calculations demonstrate that the charge transport in the zero Hall plateau state is conducted by two counter-propagating edge states that arise from the combined effects of Landau levels and large Zeeman effect in strong magnetic fields. Our result demonstrates the intricate interplay among intrinsic magnetic order, external magnetic field, and nontrivial band topology in MnBi2Te4.",2001.08401v2 2020-04-14,Highly Conducting Spaced TiO$_2$ Nanotubes Enable Defined Conformal Coating with Nanocrystalline Nb$_2$O$_5$ and High Performance Supercapacitor Applications,"In this work, we report on the electrochemical behavior of nitrided spaced TiO$_2$ nanotubes conformally coated with a nanocrystalline Nb$_2$O$_5$ layer and find for these hierarchical structures an excellent supercapacitor performance. Highly aligned conductive 1D electrodes were obtained by a three step process: i) growth of self-organized nanotubes with defined and adjustable intertube spacing, ii) conformal Nb$_2$O$_5$ decoration in the tube interspace (while providing full electrolyte access to the entire active area), and iii) high temperature nitridation. Key is the growth of a nanotube array with regular tube-to-tube interspacing that enables an optimized decoration with secondary materials such as Nb$_2$O$_5$. We observe an increase in electrode capacitance from 158 $\mu$F cm-2 for bare TiO$_2$ NTs, to 1536 $\mu$F cm-2 for TiO$_2$/Nb$_2$O$_5$ NTs, to finally 37 mF cm-2 for Nb$_2$O$_5$ decorated and then nitrided nanotubes. This drastic increase can be ascribed firstly to the defined spacing established between the tube arrays that then allows for a conformal coating with a secondary active coating. Secondly, nitridation causes a drastic increase of the electron conductivity of the entire scaffold and thus reduces resistive losses.",2005.01603v1 2020-10-13,"High-pressure synthesis of Ba$_2$RhO$_4$, a rhodate analogue of the layered perovskite Sr-ruthenate","A new layered perovskite-type oxide Ba$_2$RhO$_4$ was synthesized by a high-pressure technique with the support of convex-hull calculations. The crystal and electronic structure were studied by both experimental and computational tools. Structural refinements for powder x-ray diffraction data showed that Ba$_2$RhO$_4$ crystallizes in a K$_2$NiF$_4$-type structure, isostructural to Sr$_2$RuO$_4$ and Ba$_2$IrO$_4$. Magnetic, resistivity, and specific heat measurements for polycrystalline samples of Ba$_2$RhO$_4$ indicate that the system can be characterized as a correlated metal. Despite the close similarity to its Sr$_2$RuO$_4$ counterpart in the electronic specific heat coefficient and the Wilson ratio, Ba$_2$RhO$_4$ shows no signature of superconductivity down to 0.16 K. Whereas the Fermi surface topology has reminiscent pieces of Sr$_2$RuO$_4$, an electron-like e$_g$-($d_{x^2-y^2}$) band descends below the Fermi level, making of this compound unique also as a metallic counterpart of the spin-orbit-coupled Mott insulator Ba$_2$IrO$_4$.",2010.06556v1 2021-02-15,Magic thickness of 25 Å makes periodic metal-insulator transitions,"Novel quantum phenomena, including high-temperature superconductivity, topological properties, and charge/spin density waves, appear in low-dimensional conductive materials. It is possible to artificially create low-dimensional systems by fabricating ultrathin films, quantum wires, or quantum dots with flat interfaces. Some experiments have been performed on ultrathin compounds of strongly correlated electron systems. However, since it is technically difficult to control multiple elements precisely, most of the properties of artificially fabricated low-dimensional compounds fall into uncharted territory. Here we show that extraordinary metal-insulator transitions that oscillate depending on the scale occur in CaRuO_3 films with a thickness of around several unit cells. We grow high-crystalline CaRuO_3 ultrathin films, whose surface roughness is controlled at 199 pm, by molecular beam epitaxy. We observe that resistivity oscillates with a magic thickness of 25 {\AA}, which changes by 3 and 9 orders of magnitude at room temperature and at low temperature, respectively. These changes are much larger than quantum size effects. We also confirm the same periodicity with photoelectron spectroscopy by etching the ultrathin film. Considering the large energy, periodicity and anisotropy, we conclude that the oscillating transitions originate from the commensurability of Mott insulation triggered by Peierls instability arising from a dual restriction on the dimensions in wavenumber space and real space. We have shown the possibility of producing new functional materials by controlling film thickness on electron correlated compounds at the picometer level.",2102.07323v1 2021-06-17,Synthesis of Murunskite Single Crystals: A Bridge Between Cuprates and Pnictides,"Numerous contemporary investigations in condensed matter physics are devoted to high temperature (high-$T_c$ ) cuprate superconductors. Despite its unique effulgence among research subjects, the enigma of the high-$T_c$ mechanism still persists. One way to advance its understanding is to discover and study new analogous systems. Here we begin a novel exploration of the natural mineral murunskite, K$_2$FeCu$_3$S$_4$, as an interpolation compound between cuprates and ferropnictides, the only known high-$T_c$ superconductors at ambient pressure. Because in-depth studies can be carried out only on single crystals, we have mastered the synthesis and growth of high quality specimens. Similar to the cuprate parent compounds, these show semiconducting behavior in resistivity and optical transmittance, and an antiferromagnetic ordering at 100 K. Spectroscopy (XPS) and calculations (DFT) concur that the sulfur 3$p$ orbitals are partially open, making them accessible for charge manipulation, which is a prerequisite for superconductivity in analogous layered structures. DFT indicates that the valence band is more cuprate-like, while the conduction band is more pnictide-like. With appropriate doping strategies, this parent compound promises exciting future developments.",2106.09555v1 2021-09-14,Creep properties and deformation mechanisms of single-crystalline $γ^\prime$-strengthened superalloys in dependence of the Co/Ni ratio,"Co-base superalloys are considered as promising high temperature materials besides the well-established Ni-base superalloys. However, Ni appears to be an indispensable alloying element also in Co-base superalloys. To address the influence of the base elements on the deformation behavior, high-temperature compressive creep experiments were performed on a single crystal alloy series that was designed to exhibit a varying Co/Ni ratio and a constant Al, W and Cr content. Creep tests were performed at 900 {\deg}C and 250 MPa and the resulting microstructures and defect configurations were characterized via electron microscopy. The minimum creep rates differ by more than one order of magnitude with changing Co/Ni ratio. An intermediate CoNi-base alloy exhibits the overall highest creep strength. Several strengthening contributions like solid solution strengthening of the $\gamma$ phase, effective diffusion coefficients or stacking fault energies were quantified. Precipitate shearing mechanisms differ significantly when the base element content is varied. While the Ni-rich superalloys exhibit SISF and SESF shearing, the Co-rich alloys develop extended APBs when the $\gamma^\prime$ phase is cut. This is mainly attributed to a difference in planar fault energies, caused by a changing segregation behavior. As result, it is assumed that the shearing resistivity and the occurring deformation mechanisms in the $\gamma^\prime$ phase are crucial for the creep properties of the investigated alloy series.",2109.06767v1 2022-06-29,Tailoring of rhenium oxidation state in ReOx thin films during reactive HiPIMS deposition process and following annealing,"Bulk rhenium trioxide (ReO3) has an unusually high electrical conductivity and, being nanosized, has promising catalytic properties. However, the production of pure ReO3 thin films is challenging due to the difficulty to stabilize rhenium in a 6+ oxidation state. Here we present a novel approach for the deposition of ReOx (x = 1.6-2.9) thin films using reactive high power impulse magnetron sputtering (r-HiPIMS) from a metallic rhenium target in a mixed Ar/O2 atmosphere. The thin films were deposited in the gas-sustained self-sputtering regime, observed during r-HiPIMS process according to current waveforms. The influence of the substrate temperature, the oxygen-to-argon flow ratio and post-annealing at 250 {\deg}C in the air for 3 h on the properties of the films were studied. The as-deposited films have an X-ray amorphous structure (a-ReOx) when deposited at room temperature while a nano-crystalline \b{eta}-ReO2 phase when deposited at elevated temperatures (150 or 250 {\deg}C). The amorphous a-ReOx can be converted into the crystalline ReO3 with a lattice parameter of 3.75 {\AA} upon annealing in the air. The surface morphology of the films is dense without detectable voids when elevated substrate temperatures are used. Various Re oxidation states are observed on the surface of the films in different ratios depending on the deposition parameters. All samples exhibit electrical resistivity on the order of 10-3 Ohmxcm and optical properties typical for thin metallic films.",2206.14665v1 2022-06-02,A mechanically strong and ductile soft magnet with extremely low coercivity,"Soft magnetic materials (SMMs) serve in electrical applications and sustainable energy supply, allowing magnetic flux variation in response to changes in applied magnetic field, at low energy loss1. The electrification of transport, households and manufacturing leads to an increase in energy consumption due to hysteresis losses2. Therefore, minimizing coercivity, which scales these losses, is crucial3. Yet, meeting this target alone is not enough: SMMs in electrical engines must withstand severe mechanical loads, i.e., the alloys need high strength and ductility4. This is a fundamental design challenge, as most methods that enhance strength introduce stress fields that can pin magnetic domains, thus increasing coercivity and hysteretic losses5. Here, we introduce an approach to overcome this dilemma. We have designed a Fe-Co-Ni-Ta-Al multicomponent alloy with ferromagnetic matrix and paramagnetic coherent nanoparticles (~91 nm size, ~55% volume fraction). They impede dislocation motion, enhancing strength and ductility. Their small size, low coherency and small magnetostatic energy create an interaction volume below the magnetic domain wall width, leading to minimal domain wall pinning, thus maintaining the soft magnetic properties. The alloy has a tensile strength of 1336 MPa at 54% tensile elongation, extremely low coercivity of 78 A/m (<1 Oe), moderate saturation magnetization of 100 Am2/kg, and high electrical resistivity of 103 {\mu}{\Omega} u Ohm cm.",2207.05686v1 2022-07-26,"Cr$_3$X$_4$ (X=Se, Te) monolayers as new platform to realize robust spin filter, spin diode and spin valve","Two-dimensional ferromagnetic (FM) half-metals are promising candidates for advanced spintronic devices with small-size and high-capacity. Motivated by recent report on controlling synthesis of FM Cr$_3$Te$_4$ nanosheet, herein, to explore the potential application in spintronics, we designed spintronic devices based on Cr$_3$X$_4$ (X=Se, Te) monolayers and investigated their spin transport properties. We found that Cr$_3$Te$_4$ monolayer based device shows spin filtering and dual spin diode effect when applying bias voltage, while Cr$_3$S$_4$ monolayer is an excellent platform to realize a spin valve. The different transport properties are primarily ascribed to the semiconducting spin channel, which is close to and away from the Fermi level in Cr$_3$Te$_4$ and Cr$_3$Se$_4$ monolayers, respectively. Interestingly, the current in monolayer Cr$_3$Se$_4$ based device also displays a negative differential resistance effect (NDRE) and a high magnetoresistance ratio (up to 2*10$^3$). Moreover, we found thermally induced spin filtering effect and NDRE in Cr$_3$Se$_4$ junction when applying temperature gradient instead of bias voltage. These theoretical findings highlight the potential of Cr$_3$X$_4$ (X=Se, Te) monolayers in spintronic applications and put forward realistic materials to realize nanosale spintronic device.",2207.12679v1 2022-10-26,Ion-beam Assisted Sputtering of Titanium Nitride Thin Films,"Titanium nitride is a material of interest for many superconducting devices such as nanowire microwave resonators and photon detectors. Thus, controlling the growth of TiN thin films with desirable properties is of high importance. In previous work on niobium nitride, ion beam-assisted sputtering (IBAS) reduced nitrogen sensitivity during deposition in tandem with an increase in nominal critical temperature. We have deposited thin films of titanium nitride by both, the conventional method of DC reactive magnetron sputtering and the IBAS method and compare their superconducting critical temperatures Tc as functions of thickness, sheet resistance, and nitrogen flow rate. We perform electrical and structural characterizations by electric transport and X-ray diffraction measurements. Compared to the conventional method of reactive sputtering, the IBAS technique has demonstrated a 10% increase in nominal critical temperature and 33% reduced sensitivity to nitrogen flow, without noticeable variation in the lattice structure. Additionally, we explore the behavior of superconducting Tc in ultra-thin films. Trends in films grown at high nitrogen concentrations follow predictions of mean-field theory in disordered films and show suppression of superconducting Tc due to geometric effects, while nitride films grown at low nitrogen concentrations strongly deviate from the theoretical models.",2210.15065v3 2023-02-14,MgF$_2$ as an effective additive for improving ionic conductivity of ceramic solid electrolytes,"As typical solid-state electrolytes (SSEs), {Na}$_{1+x}${Zr}$_2${Si}$_{x}${P}$_{3-x}${O}$_{12}$ NASICONs provide an ideal platform for solid-state batteries (SSBs) that display higher safety and accommodate higher energy densities. The critical points for achieving SSBs with higher efficiencies are to improve essentially the ionic conductivity and to reduce largely the interfacial resistance between SSEs and cathode materials, which would necessitate extremely high level of craftsmanship and high-pressure equipment. An alternative to higher-performance and lower-cost SSBs is additive manufacturing. Here, we report on an effective additive, MgF$_2$, which was used in synthesizing NASICONs, resulting in SSEs with fewer defects and higher performance. With an addition of mere 1 wt$\%$ MgF$_2$ additive, the total room-temperature ionic conductivity of the NASICON electrolyte reaches up to 2.03 mS cm$^{-1}$, improved up to $\sim$ 181.3$\%$, with an activation energy of 0.277 eV. Meanwhile, the stability of the Na plating/stripping behavior in symmetric cells increases from 236 to 654 h. We tried to reveal the microscopic origins of the higher ionic conductivity of MgF$_2$-doped NASICONs by comprehensive in-house characterizations. Our study discovers a novel MgF$_2$ additive and provides an efficient way to prepare higher-performance SSEs, making it possible to fabricate lower-cost SSBs in industries.",2302.07264v1 2023-07-03,Low temperature dynamic polaron liquid in a manganite exhibiting colossal magnetoresistance,"Polarons - fermionic charge carriers bearing a strong companion lattice deformation - exhibit a natural tendency for self-localization due to the recursive interaction between electrons and the lattice. While polarons are ubiquitous in insulators, how they evolve in transitions to metallic and superconducting states in quantum materials remains an open question. Here, we use resonant inelastic x-ray scattering (RIXS) to track the electron-lattice coupling in the colossal magneto-resistive bi-layer manganite La$_{1.2}$Sr$_{1.8}$Mn$_2$O$_7$ across its metal-to-insulator transition. The response in the insulating high-temperature state features harmonic emissions of a dispersionless oxygen phonon at small energy transfer. Upon cooling into the metallic state, we observe a drastic redistribution of spectral weight from the region of these harmonic emissions to a broad high energy continuum. In concert with theoretical calculations, we show that this evolution implies a shift in electron-lattice coupling from static to dynamic lattice distortions that leads to a distinct polaronic ground state in the low temperature metallic phase - a dynamic polaron liquid.",2307.00718v3 2023-09-24,FeCo Nanowire-Strontium Ferrite Powder Composites for Permanent Magnets with High-Energy Products,"Due to the issues associated with rare-earth elements, there arises a strong need for magnets with properties between those of ferrites and rare-earth magnets that could substitute the latter in selected applications. Here, we produce a high remanent magnetization composite bonded magnet by mixing FeCo nanowire powders with hexaferrite particles. In the first step, metallic nanowires with diameters between 30 and 100 nm and length of at least 2 {\mu}m are fabricated by electrodeposition. The oriented as-synthesized nanowires show remanence ratios above 0.76 and coercivities above 199 kA/m and resist core oxidation up to 300 {\deg}C due to the existence of a > 8 nm thin oxide passivating shell. In the second step, a composite powder is fabricated by mixing the nanowires with hexaferrite particles. After the optimal nanowire diameter and composite composition are selected, a bonded magnet is produced. The resulting magnet presents a 20% increase in remanence and an enhancement of the energy product of 48% with respect to a pure hexaferrite (strontium ferrite) magnet. These results put nanowire-ferrite composites at the forefront as candidate materials for alternative magnets for substitution of rare earths in applications that operate with moderate magnet performance.",2309.13724v1 2023-11-01,Transport and electrical properties of cryogenic thermoelectric FeSb2: the effect of isoelectronic and hole doping,"Thermoelectric materials operating at cryogenic temperatures are in high demand for efficient cooling and power generation in applications ranging from superconductors to quantum computing. The narrow band-gap semiconductor FeSb2, known for its colossal Seebeck coefficient, holds promise for such applications, provided its thermal conductivity value can be reduced. This study investigates the impact of isoelectronic substitution (Bi) and hole doping (Pb) at the Sb site on the transport properties of FeSb2, with a particular focus on thermal conductivity (\k{appa}). Polycrystalline FeSb2 powder, along with Bi- and Pb-doped samples, were synthesized using a simple co-precipitation approach, followed by thermal treatment in an H2 atmosphere. XRD and SEM analysis confirms the formation of the desired phase pre- and post-consolidation using spark plasma sintering (SPS). The consolidation process resulted in a high compaction density and the formation of submicrometer-sized grains, as substantiated by electron backscattered diffraction (EBSD) analysis. Substituting 1% of Bi and Pb at the Sb site successfully suppressed the thermal conductivity (\k{appa}) from ~15 W/m-K in pure FeSb2 to ~10 and ~8.7 W/m-K, respectively. Importantly, resistivity measurements revealed a metal-to-insulator transition at around 6.5 K in undoped FeSb2 and isoelectronically Bi-substituted FeSb2, suggesting the existence of metallic surface states and provides valuable evidence for the perplexing topological behavior exhibited by FeSb2.",2311.00326v1 2023-12-13,Computational design of NDR tunnel diodes with high peak-to-valley current ratio based on two-dimensional cold metals: The case of NbSi$_2$N$_4$/HfSi$_2$N$_4$/NbSi$_2$N$_4$ lateral heterojunction diode,"Cold metals have recently gained attention as a promising platform for innovative devices, such as tunnel diodes with negative differential resistance (NDR) and field-effect transistors with subthreshold swings below the thermionic limit. Recently discovered two-dimensional (2D) MA$_2$Z$_4$ (M = Ti, Zr, Hf, Nb, Ta; A = Si, Ge; Z = N, P) compounds exhibit both cold metallic and semiconducting behavior. In this work, we present a computational study of lateral heterojunction tunnel diodes based on 2D NbSi$_2$N$_4$ and HfSi$_2$N$_4$ compounds. Employing density functional theory combined with a nonequilibrium Green function method, we investigate the current-voltage ($I$-$V$) characteristics of lateral tunnel diodes with varying barrier thicknesses in both zigzag and armchair orientations. We find that tunnel diodes in the zigzag orientation exhibit significantly higher peak current densities, while those in the armchair orientation display larger peak-to-valley current ratios (PVCRs) compared to the zigzag orientation. Our findings suggest that MA$_2$Z$_4$ materials are promising candidates for realizing NDR tunnel diodes with high PVCR values, which could have potential applications in memory, logic circuits, and other electronic devices.",2312.08473v2 2024-01-29,Increasing the Collection Efficiency in Selenium Thin-Film Solar Cells Using a Closed-Space Annealing Strategy,"Elemental selenium is a promising wide-bandgap ($E_\mathrm{G}\approx$ 1.95 eV) photovoltaic material for the next generation of thin-film solar cells. To realize high-efficiency selenium solar cells, it is crucial to optimize the crystallization process of the selenium thin-film photoabsorber. However, the high vapor pressure of selenium restricts the processing conditions to a compromise between the growth of large crystal grains and the formation of pinholes. In this study, we introduce a closed-space annealing (CSA) strategy designed to suppress the sublimation of selenium, enabling thermal annealing processes at higher temperatures and for longer periods of time. As a result, we consistently improve carrier collection and the overall photovoltaic device performance in our selenium solar cells. By characterizing the carrier dynamics in our devices, we conclude that the observed improvements result from a reduction in charge transfer resistance rather than an increase in carrier diffusion length. The CSA strategy is a promising method for controlling surface morphology and roughness without reducing crystal grain sizes, which paves the way for further advancements in the efficiency and reproducibility of selenium thin-film solar cells.",2401.15936v1 2024-02-10,Cylindrical compression of thin wires by irradiation with a Joule-class short pulse laser,"Equation of state measurements at Jovian or stellar conditions are currently conducted by dynamic shock compression driven by multi-kilojoule multi-beam nanosecond-duration lasers. These experiments require precise design of the target and specific tailoring of the spatial and temporal laser profiles to reach the highest pressures. At the same time, the studies are limited by the low repetition rate of the lasers. Here, we show that by the irradiation of a thin wire with single beam Joule-class short-pulse laser, a converging cylindrical shock is generated compressing the wire material to conditions relevant for the above applications. The shockwave was observed using Phase Contrast Imaging employing a hard X-ray Free Electron Laser with unprecedented temporal and spatial sensitivity. The data collected for Cu wires is in agreement with hydrodynamic simulations of an ablative shock launched by a highly-impulsive and transient resistive heating of the wire surface. The subsequent cylindrical shockwave travels towards the wire axis and is predicted to reach a compression factor of 9 and pressures above 800 Mbar. Simulations for astrophysical relevant materials underline the potential of this compression technique as a new tool for high energy density studies at high repetition rates.",2402.06983v1 2024-03-04,Quantum Hall Transport Measurements of Lateral p-n Junctions Formed via Precise Spatial Photodoping of Graphene/hBN Heterostructures,"Heterostructures composed of 2-dimensional (2D) materials are spatially dope in-operando to modify devices for custom functionalities, such as lateral p-n-p junctions. After optically photodoping an hBN/Graphene/hBN heterostructure, detailed magnetotransport measurements including quantum Hall transport show several clear electronic regimes. In the p+-p-p+ and n-n+-n configurations, we see clear quantization of the longitudinal resistance. Using the Landauer-Buttiker model we elucidate the nature of the electrostatic profile at the interface between the doped regions. In the p-n-p configuration, due to the heavily graded junction profile that completely separates the p- and n-Landau level edge states from interacting, an ""insulating"" state is observed that is not common and has not been measured in previous quantum Hall transport measurements of graphene pnJ devices in high magnetic fields. This insulating state is promising as the basis for a high-performance graphene switching device with a good ON/OFF ratio. In principle, these doping and measurement techniques can be applied to any other 2D heterostructure encapsulated within an hBN sandwich to understand the quality of the electrostatic interface between doped regions.",2403.01998v1 2020-12-05,"A15 Nb$_3$Si -- A ""high"" Tc superconductor synthesized at a pressure of one megabar and metastable at ambient conditions","A15 Nb$_3$Si is, until now, the only high temperature superconductor produced at high pressure (~110 GPa) that has been successfully brought back to room pressure conditions in a metastable condition. Based on the current great interest in trying to create metastable-at-room-pressure high temperature superconductors produced at high pressure, we have restudied explosively compressed A15 Nb$_3$Si and its production from tetragonal Nb$_3$Si. First, diamond anvil cell pressure measurements up to 88 GPa were performed on explosively compressed A15 Nb$_3$Si material to trace Tc as a function of pressure. Tc is suppressed to ~ 5.2 K at 88 GPa. Then, using these Tc (P) data for A15 Nb$_3$Si, pressures up to 92 GPa were applied at room temperature (which increased to 120 GPa at 5 K) on tetragonal Nb$_3$Si. Measurements of the resistivity gave no indication of any A15 structure production, i.e., no indications of the superconductivity characteristic of A15 Nb$_3$Si. This is in contrast to the explosive compression (up to P~110 GPa) of tetragonal Nb$_3$Si, which produced 50-70% A15 material, Tc = 18 K at ambient pressure, in a 1981 Los Alamos National Laboratory experiment. Our theoretical calculations show that A15 Nb$_3$Si has an enthalpy vs the tetragonal structure that is 0.07 eV/atom smaller at 100 GPa, implying that the accompanying high temperature (1000 deg C) caused by explosive compression is necessary to successfully drive the reaction kinetics of the tetragonal -> A15 Nb$_3$Si structural transformation. Annealing experiments on the A15 explosively compressed material reaching time scales of 39 years are consistent with this viewpoint.",2012.02905v2 2006-03-17,Second Core Formation and High Speed Jets: Resistive MHD Nested Grid Simulations,"The stellar core formation and high speed jets driven by the formed core are studied by using three-dimensional resistive MHD nested grid simulations. Starting with a Bonnor-Ebert isothermal cloud rotating in a uniform magnetic field, we calculate the cloud evolution from the molecular cloud core (n = 10^6 cm^-3, r_c = 4.6 times 10^4 AU) to the stellar core (n \simeq 10^23 cm^-3, r_c \simeq 1 solar radius). We resolve cloud structure over 7 orders of magnitude in spatial extent and over 17 orders of magnitude in density contrast. For comparison, we calculate two models: resistive and ideal MHD models. Both models have the same initial condition, but the former includes dissipation process of magnetic field while the latter does not. The magnetic fluxes in resistive MHD model are extracted from the first core during 10^12 cm^-3 < n < 10^16 cm^-3 by Ohmic dissipation. Magnetic flux density of the formed stellar core (n \simeq 10^20 cm^-3) in resistive MHD model is two orders of magnitude smaller than that in ideal MHD model. Since magnetic braking is less effective in resistive MHD model, rapidly rotating stellar core (the second core) is formed. After stellar core formation, the magnetic field of the core is largely amplified both by magneto-rotational instability and the shearing motion between the stellar core and ambient medium. As a consequence, high speed (simeq 45 km,s^-1) jets are driven by the second core, which results in strong mass ejection. A cocoon-like structure around the second core also forms with clear bow shocks.",0603456v1 2018-05-07,Appearance of ferromagnetism property for Si nano-polycrystalline body and vanishing of electrical resistances at local high frequencies,"Reduction in the skin effect for the sintered Si nanopolycrystalline body as an electricity conductor at a high frequency due to its nano-structure was studied. Singular vanishing of electrical resistances near a local high magnetic harmonic frequency of a few MHz was observed. This phenomenon has not been observed for conventional ferromagnetic metals. The measured electrical resistances changed to almost 0 m{\Omega} at room temperature. At the same time, negative resistance of the sintered Si nano-polycrystalline body was observed. It will be applicable to electronic transmittance lines or semiconductors. Numerical calculation was also performed on the electrical resistance with frequency dependency while considering the electric field and magnetic field in the sintered Si nanopolycrystalline body. The calculation could explain the variation of the relative permittivity of the Si nanopolycrystalline and the phenomenon for vanishing the resistivity at frequency of MHz theoretically. Reduced Si nanoparticles from SiO2 powder were synthesized by laser ablation in liquid. A Si nano-polycrystalline body made of the reduced Si nanoparticles was fabricated. It was found by measuring the magnetization property of the body that the sintered Si nano-polycrystalline body has ferromagnetism. High-density dangling bonds cause the sintered Si nanopolycrystalline to have ferromagnetism. In this study, the density of the unpaired electrons in the sintered Si nanopolycrystalline was observed using ESR. It has been clarified that the Si nanopowder and the sintered Si nanopolycrystalline have numerous dangling bonds. Both densities of the dangling bonds were evaluated.",1805.02312v1 2019-03-26,The micro-RWELL layouts for high particle rate,"The $\mu$-RWELL is a single-amplification stage resistive Micro-Pattern Gaseous Detector (MPGD). The detector amplification element is realized with a single copper-clad polyimide foil micro-patterned with a blind hole (well) matrix and embedded in the readout PCB through a thin Diamond-Like-Carbon (DLC) sputtered resistive film. The introduction of the resistive layer, suppressing the transition from streamer to spark, allows to achieve large gains ($\geq$10$^4$) with a single amplification stage, while partially reducing the capability to stand high particle fluxes. The simplest resistive layout, designed for low-rate applications, is based on a single-resistive layer with edge grounding. At high particle fluxes this layout suffers of a non-uniform response. In order to get rid of such a limitation different current evacuation geometries have been designed. In this work we report the study of the performance of several high rate resistive layouts tested at the CERN H8-SpS and PSI $\pi$M1 beam test facilities. These layouts fulfill the requirements for the detectors at the HL-LHC and for the experiments at the next generation colliders FCC-ee/hh and CepC.",1903.11017v2 2018-04-15,$\mathrm{Co_2Fe_{1-x}Cr_xSi}$ Heusler Alloys : A promising material for spintronics application,"In this article, we investigated the effect of Cr substitution in place of Fe on the structural, magnetic and transport properties of $\mathrm{Co_2FeSi}$ alloy. A comprehensive structural analysis is done using X-ray diffraction (XRD) and extended X-ray absorption fine structure (EXAFS) spectroscopy. Quaternary Heusler compounds $\mathrm{Co_2Fe_{1-x}Cr_xSi}$ with Cr content (x = 0.1, 0.3, 0.5) were found to crystallize in cubic structure. The synchrotron based EXAFS studies reveal that the anti-site disorder increases with the increase in Cr concentration. The saturation magnetization values in all the alloys are found to be less than those expected from the Slater-Pauling rule, which may be due to the some inherent disorder. A detailed resistivity analysis in the temperature range of 5-300 K is done, taking into account different scattering mechanisms. The residual resistivity ratio is found to decrease with increasing Cr concentration. A disorder induced resistivity minimum due to weak localization effect is seen for x = 0.5. The resistivity measurements also indicate that the half-metallic character survives upto 100 K for x = 0.1, whereas the alloys with x= 0.3 and 0.5 show signature of half- metallic nature even at higher temperatures. First principles calculation done with a more robust exchange correlation functional (namely HSE-06) confirms the half metallicity in the entire concentration range. Theoretically simulated band gap and magnetic moments compliment the experimental findings and are compared wherever possible. All these properties make $\mathrm{Co_2Fe_{1-x}Cr_xSi}$ a promising material for spintronics application.",1804.05321v1 2021-10-16,Giant magnetoresistance and topological Hall effect in the EuGa4 antiferromagnet,"We report on systematic temperature- and magnetic field-dependent studies of the EuGa$_4$ binary compound, which crystallizes in a centrosymmetric tetragonal BaAl$_4$-type structure with space group $I4/mmm$. The electronic properties of EuGa$_4$ single crystals, with an antiferromagnetic (AFM) transition at $T_\mathrm{N} \sim 16.4$ K, were characterized via electrical resistivity and magnetization measurements. A giant nonsaturating magnetoresistance was observed at low temperatures, reaching $\sim 7 \times 10^4$ % at 2 K in a magnetic field of 9 T. In the AFM state, EuGa$_4$ undergoes a series of metamagnetic transitions in an applied magnetic field, clearly manifested in its field-dependent electrical resistivity. Below $T_\mathrm{N}$, in the $\sim$4-7 T field range, we observe also a clear hump-like anomaly in the Hall resistivity which is part of the anomalous Hall resistivity. We attribute such a hump-like feature to the topological Hall effect, usually occurring in noncentrosymmetric materials known to host topological spin textures (as e.g., magnetic skyrmions). Therefore, the family of materials with a tetragonal BaAl$_4$-type structure, to which EuGa$_4$ and EuAl$_4$ belong, seems to comprise suitable candidates on which one can study the interplay among correlated-electron phenomena (such as charge-density wave or exotic magnetism) with topological spin textures and topologically nontrivial bands.",2110.08522v1 2016-01-09,Field-induced resistivity plateau and unsaturated negative magnetoresistance in topological semimetal TaSb2,"Several prominent transport properties have been identified as key signatures of topologicalmaterials. One is the resistivity plateau at low temperatures as observed in several topological insulators (TIs), another is the negative magnetoresistance (MR) when the applied magnetic field is parallel to the current direction as observed in several topological semimetals (TSMs) including Dirac semimetals (DSMs) and Weyl semimetals (WSMs). Usually, these two exotic phenomena emerge in distinct materials with or without time reversal symmetry (TRS), respectively. Here we report the discovery of a new member in TSMs, TaSb2, which clearly exhibits both of these phenomena in a single material. This compound crystallizes in a base-centered monoclinic, centrosymmetric structure, and is metallic with a low carrier density in the zero field. While applying magnetic field it exhibits insulating behavior before appearance of a resistivity plateau below Tc =13 K. In the plateau regime, the ultrahigh carrier mobility and extreme magnetoresistance (XMR) for the field perpendicular to the current are observed as in DSMs and WSMs, in addition to a quantum oscillation behavior with non-trivial Berry phases. In contrast to the most known DSMs and WSMs, the negative MR in TaSb2 does not saturate up to 9 T, which, together with the almost linear Hall resistivity, manifests itself an electron-hole non-compensated TMS. These findings indicate that the resistivity plateau could be a generic feature of topology-protected metallic states even in the absence of TRS and compatible with the negative MR depending on the field direction. Our experiment extends a materials basis represented by TaSb2 as a new platform for future theoretical investigations and device applications of topological materials.",1601.02062v1 2011-01-31,Encapsulation and Electronic Control of Epitaxial Graphene by Photosensitive Polymers and UV light,"Electronic devices using epitaxial graphene on Silicon Carbide require encapsulation to avoid uncontrolled doping by impurities deposited in ambient conditions. Additionally, interaction of the graphene monolayer with the substrate causes relatively high level of electron doping in this material, which is rather difficult to change by electrostatic gating alone. Here we describe one solution to these problems, allowing both encapsulation and control of the carrier concentration in a wide range. We describe a novel heterostructure based on epitaxial graphene grown on silicon carbide combined with two polymers: a neutral spacer and a photoactive layer that provides potent electron acceptors under UV light exposure. Unexposed, the same double layer of polymers works well as capping material, improving the temporal stability and uniformity of the doping level of the sample. By UV exposure of this heterostructure we controlled electrical parameters of graphene in a non-invasive, non-volatile, and reversible way, changing the carrier concentration by a factor of 50. The electronic properties of the exposed SiC/ graphene/polymer heterostructures remained stable over many days at room temperature, but heating the polymers above the glass transition reversed the effect of light. The newly developed photochemical gating has already helped us to improve the robustness (large range of quantizing magnetic field, substantially higher opera- tion temperature and significantly enhanced signal-to-noise ratio due to significantly increased breakdown current) of a graphene resistance standard to such a level that it starts to compete favorably with mature semiconductor heterostructure standards. [2,3]",1101.6014v1 2020-11-20,Phase Transitions in Germanium Telluride Nanoparticle Phase-Change Materials Studied by Time-Resolved X-Ray Diffraction,"Germanium telluride (GeTe), a phase-change material, is known to exhibit four different structural phases: three at room temperature (one amorphous and two crystalline, $\alpha$ and $\gamma$) and one at high temperature (crystalline $\beta$). Because transitions between the amorphous and crystalline phases lead to significant changes in material properties (e.g., refractive index and resistivity), GeTe has been investigated as a phase-change material for photonics, thermoelectrics, ferroelectrics, and spintronics. Consequently, the temperature-dependent phase transitions in GeTe have been studied for bulk and thin-film GeTe, both fabricated by sputtering. Colloidal synthesis of nanoparticles offers a more flexible fabrication approach for amorphous and crystalline GeTe. These nanoparticles are known to exhibit size-dependent properties, such as an increased crystallization temperature for the amorphous-to-$\alpha$ transition in sub-10\,nm GeTe particles. The $\alpha$-to-$\beta$ phase transition is also expected to vary with size, but this effect has not yet been investigated for GeTe. Here, we report time-resolved X-ray diffraction of GeTe nanoparticles with different diameters and from different synthetic protocols. We observe a non-volatile amorphous-to-$\alpha$ transition between 210$^{\circ}$C and 240$^{\circ}$C and a volatile $\alpha$-to-$\beta$ transition between 370$^{\circ}$C and 420$^{\circ}$C. The latter transition was reversible and repeatable. While the transition temperatures are shifted relative to the values known for bulk GeTe, the nanoparticle-based samples still exhibit the same structural phases reported for sputtered GeTe. Thus, colloidal GeTe maintains the same general phase behavior as bulk GeTe while allowing for more flexible and accessible fabrication. Therefore, nanoparticle-based GeTe films show great potential for applications, such as in active photonics.",2011.10633v1 2022-08-23,Electrochemical investigation of MoSeTe as an anode for sodium-ion batteries,"Sodium ion batteries (SIBs) are considered as an efficient alternative for lithium-ion batteries (LIBs) owing to the natural abundance and low cost of sodium than lithium. In this context, the anode materials play a vital role in rechargeable batteries to acquire high energy and power density. In order to demonstrate transition metal dichalcogenide (TMD) as potential anode materials, we have synthesized MoSeTe sample by conventional flux method, and the structure and morphology are characterized using x-ray diffraction (XRD), field-emission scanning electron microscopy (FESEM), transmission electron microscopy (TEM), and Raman spectroscopy. These characterisations confirm the hexagonal crystal symmetry with p63/mmc space group and layered morphology of MoSeTe. We investigate the electrochemical performance of a MoSeTe as a negative electrode (anode) for SIBs in the working potential range of 0.01 to 3.0~V. In a half-cell configuration, the MoSeTe as an anode and Na metal as counter/reference electrode exhibits significant initial specific discharge capacities of around 475 and 355 mAhg$^{-1}$ at current densities of 50 and 100 mAg$^{-1}$, respectively. However, the capacity degraded significantly like $\approx$200~mAhg$^{-1}$ in 2nd cycle, but having $\approx$100\% Coulombic efficiency, which suggest for further modification in this material to improve its stability. The cyclic voltammetry (CV) study reveals the reversibility of the material after 1st cycle, resulting no change in the initial peak positions. The electrochemical impedance spectroscopy (EIS) measurements affirms the smaller charge transfer resistance of fresh cells than the cells after 10th cycle. Moreover, the extracted diffusion coefficient is found to be of the order of 10$^{-14}$ cm$^2$s$^{-1}$.",2208.10911v1 2024-05-13,"Reducing the oxygen contamination in conductive (Ti,Zr)N coatings via RF-bias assisted reactive sputtering","Ternary transition metal nitride coatings are promising for many applications as they can offer improved hardness and oxidation resistance compared to binary counterparts. A common challenge in the deposition of functional nitride thin films is oxygen contamination. Even low amounts of oxygen contamination can adversely affect the functional properties of the thin films. Here, we present a practical approach for the growth of virtually oxygen-free (Ti, Zr)N thin films. To cover the complete compositional range of (Ti,Zr)N coatings we employ combinatorial reactive co-sputtering. The depositions are carried out with or without applying a low-power radio-frequency (RF) bias voltage to the substrate holder to study the possibility of decelerating energetic oxygen ions and effectively reducing oxygen contamination in the growing film. High-throughput structural analysis and functional property mapping are used to elucidate the synthesis-property relationships. The structural analysis indicates solid solution formation over the entire compositional range, as evidenced by Vegardian lattice scaling, regardless of the applied RF substrate bias. Irrespective of the composition of the films, the application of RF substrate bias leads to a dramatic reduction of oxygen contamination, as demonstrated by X-ray photoelectron spectroscopy (XPS) depth-profile mapping. This is reflected in a significant improvement in the films' conductivity and hardness. We demonstrate that the reduction in oxygen contamination is intrinsic to the process and not due to changes in the microstructure. The approach presented here is applicable to both conductive and insulating substrates and provides a practical route to synthesize nitride thin films with improved purity that can be applied in standard sputter chambers and on many different material systems.",2405.07789v1 2018-11-03,"Pressure-induced Insulator to Metal Transition of Mixed Valence Compound Ce(O,F)SbS$_{2}$","Transport properties of Ce$_{0.85}$F0.15SbS$_{2}$ and undoped CeOSbS$_{2}$ under high pressure were investigated experimentally and theoretically. Electrical resistivity measurements of the Ce$_{0.85}$F0.15SbS$_{2}$ single crystals were performed under various high pressures using a diamond anvil cell with boron-doped diamond electrodes. The samples showed the insulator to metal transition by applying high pressure up to 30-40 GPa. On the other hand, the undoped CeOSbS$_{2}$ showed almost same transport property with the F-doped sample under high pressure. The valence state analysis using X-ray photoelectron spectroscopy revealed a simple valence state of Ce3+ in Ce$_{0.85}$F0.15SbS$_{2}$ and mixed valence state between Ce3+ and Ce4+ in undoped CeOSbS$_{2}$. The valence fluctuation in Ce carried out the comparable transport nature in the both samples. A band calculation suggests that the undoped CeOSbS$_{2}$ could be metallic under high pressure of 30 GPa in accordance with the experimental results. A superior thermoelectric property of power factor in CeOSbS$_{2}$ was estimated under high pressure around 20 GPa in comparison with that of ambient pressure.",1811.01151v1 2020-10-22,A photogrammetric method for target monitoring inside the MEG II detector,"An automatic target monitoring method based on photographs taken by a CMOS photo-camera has been developed for the MEG II detector. The technique could be adapted for other fixed-target experiments requiring good knowledge of their target position to avoid biases and systematic errors in measuring the trajectories of the outcoming particles. A CMOS-based, high resolution, high radiation tolerant and high magnetic field resistant photo-camera was mounted inside the MEG II detector at the Paul Scherrer Institute (Switzerland). MEG II is used to search for lepton flavour violation in muon decays. The photogrammetric method's challenges, affecting measurements of low momentum particles' tracks, are high magnetic field of the spectrometer, high radiation levels, tight space constraints, and the need to limit the material budget in the tracking volume. The camera is focused on dot pattern drawn on the thin MEG II target, about 1 m away from the detector endcaps where the photo-camera is placed. Target movements and deformations are monitored by comparing images of the dots taken at various times during the measurement. The images are acquired with a Raspberry board and analyzed using a custom software. Global alignment to the spectrometer is guaranteed by corner cubes placed on the target support. As a result, the target monitoring fulfils the needs of the experiment.",2010.11576v2 2021-02-04,Disorder-robust high-field superconducting phase of FeSe single crystals,"When exposed to high magnetic fields, certain materials manifest an exotic superconducting (SC) phase that has attracted considerable attention. A proposed explanation for the origin of the high-field SC phase is the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state. This state is characterized by inhomogeneous superconductivity, where the Cooper pairs have finite center-of-mass momenta. Recently, the high-field SC phase was observed in FeSe, and it was deemed to originate from the FFLO state. Here, we synthesize FeSe single crystals with different levels of disorder. The level of disorder is expressed by the ratio of the mean free path to the coherence length and ranges between 35 and 1.2. The upper critical field \textit{B}$_{\rm{c}2}$ was obtained by both resistivity and magnetic torque measurements over a wide range of temperatures, which went as low as $\sim$0.5 K, and magnetic fields, which went up to $\sim$38 T along the \textit{c} axis and in the \textit{ab} plane. In the high-field region parallel to the \textit{ab} plane, an unusual SC phase was confirmed in all the crystals, and the phase was found to be robust against disorder. This result suggests that the high-field SC phase in FeSe is not a conventional FFLO state.",2102.02353v2 2021-03-03,On the early stages of precipitation during direct ageing of Alloy 718,"The Ni-based superalloy Alloy 718 is used in aircraft engines as high-pressure turbine discs and must endure challenging demands on high-temperature yield strength, creep-, and oxidation-resistance. Nanoscale $\gamma^{\prime}$- and $\gamma^{\prime \prime}$-precipitates commonly found in duplet and triplet co-precipitate morphologies provide high-temperature strength under these harsh operating conditions. Direct ageing of Alloy 718 is an attractive alternative manufacturing route known to increase the yield strength at 650 $^{\deg}$C by at least +10 $\%$, by both retaining high dislocation densities and changing the nanoscale co-precipitate morphology. However, the detailed nucleation and growth mechanisms of the duplet and triplet co-precipitate morphologies of $\gamma^{\prime}$ and $\gamma^{\prime \prime}$ during the direct ageing process remain unknown. We provide a correlative high-resolution microscopy approach using transmission electron microscopy, high-angle annular dark-field imaging, and atom probe microscopy to reveal the early stages of precipitation during direct ageing of Alloy 718. Quantitative stereological analyses of the $\gamma^{\prime}$- and $\gamma^{\prime \prime}$-precipitate dispersions as well as their chemical compositions have allowed us to propose a qualitative model of the microstructural evolution. It is shown that fine $\gamma^{\prime}$- and $\gamma^{\prime \prime}$-precipitates nucleate homogeneously and grow coherently. However, $\gamma^{\prime \prime}$-precipitates also nucleate heterogeneously on dislocations and experience accelerated growth due to Nb pipe diffusion. Moreover, the co-precipitation reactions are largely influenced by solute availability and the potential for enrichment of Nb and rejection of Al+Ti.",2103.02763v1 2022-06-25,High-Mobility Tri-Gate $β$-Ga$_2$O$_3$ MESFETs with a Power Figure of Merit over 0.9 GW/cm$^2$,"In this letter, fin-shape tri-gate $\beta$-Ga$_{2}$O$_{3}$ lateral MESFETs are demonstrated with a high power figure of merit of 0.95 GW/cm$^{2}$ - a record high for any $\beta$-Ga$_{2}$O$_{3}$ transistor to date. A low-temperature undoped buffer-channel stack design is developed which demonstrates record high Hall and drift electron mobilities in doped $\beta$-Ga$_{2}$O$_{3}$ channels allowing for low ON resistances R$_{ON}$ in $\beta$-Ga$_{2}$O$_{3}$ MESFETs. Fin-widths (W$_{fin}$) were 1.2-1.5 $\mu$m and there were 25 fins (N$_{fin}$) per device with a trench depth of $\sim$1$\mu$m. A $\beta$-Ga$_2$O$_3$ MESFET with a source-drain length of 6.4 $\mu$m exhibits a high ON current (187 mA/mm), low R$_{ON}$ (20.5 $\Omega$.mm) and a high average breakdown field (4.2 MV/cm). All devices show very low reverse leakage until catastrophic breakdown for breakdown voltages scaled from 1.1kV to $\sim$3kV. This work demonstrates the potential of channel engineering in improving $\beta$-Ga$_{2}$O$_{3}$ device performance toward lower conduction losses for low-to-medium voltage applications.",2206.12539v2 2023-10-22,Pressure-induced volumetric negative thermal expansion in CoZr2 superconductor,"We investigate the thermal expansion and superconducting properties of a CuAl2-type (tetragonal) superconductor CoZr2 under high pressures. We perform high-pressure synchrotron X-ray diffraction in a pressure range of 2.9 GPa < P < 10.4 GPa and discover that CoZr2 exhibits volumetric negative thermal expansion under high pressures. Although the uniaxial positive thermal expansion (PTE) along the a-axis is observed under ambient pressure, that is suppressed by pressure, while the large uniaxial negative thermal expansion (NTE) along the c-axis is maintained under the pressure regime. As a result of a combination of the suppressed uniaxial PTE along the a-axis and uniaxial NTE along the c-axis, volumetric negative thermal expansion is achieved under high pressure in CoZr2. The mechanisms of volumetric NTE would be based on the flexible crystal structure caused by the soft Co-Co bond as seen in the iso-structural compound FeZr2, which exhibits uniaxial NTE along the c-axis. We also perform high-pressure electrical resistance measurements of CoZr2 to confirm the presence of superconductivity under the examined pressure regime in the range of 0.03 GPa < P < 41.9 GPa. We confirm the presence of superconductivity under all pressures and observe dome-like shape pressure dependence of superconducting transition temperature. Because of the coexistence of two phenomena, which are volumetric NTE and superconductivity, in CoZr2 under high pressure, the coexistence would be achievable under ambient pressure by tuning chemical compositions after our present observation.",2310.14254v2 2023-10-22,Superconductivity in the high-entropy ceramics Ti0.2Zr0.2Nb0.2Mo0.2Ta0.2Cx with possible nontrivial band topology,"Topological superconductors have drawn significant interest from the scientific community due to the accompanying Majorana fermions. Here, we report the discovery of electronic structure and superconductivity in high-entropy ceramics Ti0.2Zr0.2Nb0.2Mo0.2Ta0.2Cx (x = 1 and 0.8) combined with experiments and first-principles calculations. The Ti0.2Zr0.2Nb0.2Mo0.2Ta0.2Cx high-entropy ceramics show bulk type-II superconductivity with Tc about 4.00 K (x = 1) and 2.65 K (x = 0.8), respectively. The specific heat jump is equal to 1.45 (x = 1) and 1.52 (x = 0.8), close to the expected value of 1.43 for the BCS superconductor in the weak coupling limit. The high-pressure resistance measurements show that a robust superconductivity against high physical pressure in Ti0.2Zr0.2Nb0.2Mo0.2Ta0.2C, with a slight Tc variation of 0.3 K within 82.5 GPa. Furthermore, the first-principles calculations indicate that the Dirac-like point exists in the electronic band structures of Ti0.2Zr0.2Nb0.2Mo0.2Ta0.2C, which is potentially a topological superconductor. The Dirac-like point is mainly contributed by the d orbitals of transition metals M and the p orbitals of C. The high-entropy ceramics provide an excellent platform for the fabrication of novel quantum devices, and our study may spark significant future physics investigations in this intriguing material.",2310.14271v1 2024-03-25,In situ growth of hydrophilic nickel-cobalt layered double hydroxides nanosheets on biomass waste-derived porous carbon for high-performance hybrid supercapacitors,"Rational design and cost-effective fabrication of layered double hydroxides (LDHs) nanosheets with extraordinary electrochemical performance is a key challenge for hybrid supercapacitors (HSCs). Herein, we report a facile in situ growth methodology to eco-friendly synthesize hydrophilic NiCo-LDHs nanosheets on biomass waste-derived porous carbon (BC) for robust high-performance HSC cathode. The in situ growth process under ultrasonication realizes the rational arrangement of NiCo-LDHs nanosheets on the surface of BC, which effectively increases the specific surface area, promotes the electronic conductivity and enhances the wettability of NiCo-LDHs nanosheets without affecting their thickness values. With the beneficial effects of ultrathin thickness of LDHs nanosheets (6.20 nm), large specific surface area (2324.1 m2 g-1), low charge transfer resistance (1.65 ohm), and high wettability with electrolyte (34-35 degree), the obtained Ni2Co1-LDHs/BC50 electrode possesses an ultra-high specific capacitance of 2390 F g-1 (956 C g-1) at 1 A g-1, which is superior to most reported values. Furthermore, an assembled Ni2Co1-LDHs/BC50//YP-80F HSC delivers a maximum specific energy of 52.47 Wh kg-1 at 375 W kg-1, and maintains a high capacitance retention of 75.9% even after 4000 cycles. This work provides a facile approach to fabricate LDHs nanosheets based cathode materials for high-performance HSCs.",2403.16506v1 1997-01-08,Coupling between phonons and intrinsic Josephson oscillations in cuprate superconductors,"The recently reported subgap structures observed in the current-voltage characteristic of intrinsic Josephson junctions in the high-T_c superconductors Tl_2Ba_2Ca_2Cu_3O_{10+\delta} and Bi_2Sr_2CaCu_2O_{8+\delta} are explained by the coupling between c-axis phonons and Josephson oscillations. A model is developed where c-axis lattice vibrations between adjacent superconducting multilayers are excited by the Josephson oscillations in a resistive junction. The voltages of the lowest structures correspond well to the frequencies of longitudinal c-axis phonons with large oscillator strength in the two materials, providing a new measurement technique for this quantity.",9701049v2 1997-07-17,Anomalous magnetotransport in wide quantum wells,"We present magneto transport experiments of quasi 3D PbTe wide quantum wells. A plateau-like structure in the Hall resistance is observed, which corresponds to the Shubnikov de Haas oscillations in the same manner as known from the quantum Hall effect. The onsets of plateaux in Rxy do not correspond to 2D filling factors but coincide with the occupation of 3D (bulk-) Landau levels. At the same time a non-local signal is observed which corresponds to the structure in Rxx and Rxy and fulfils exactly the Onsager-Casimir relation (Rij,kl(B) = Rkl,ij(-B)). We explain the behaviour in terms of edge channel transport which is controlled by a permanent backscattering across a system of ""percolative EC - loops"" in the bulk region. Long range potential fluctuations with an amplitude of the order of the subband splitting are explained to play an essential role in this electron system.",9707173v1 1997-07-18,Edge Channel Dominated Magnetotransport in PbTe Wide Parabolic Quantum Wells,"In PbTe wide parabolic quantum wells (WPQW) a plateau-like structure is observed in the Hall resistance, which corresponds to the Shubnikov-de Haas oscillations in the same manner as known from the quantum Hall effect. At the same time a non-local signal is observed which corresponds to the structure in Rxx and Rxy. We find a striking correspondence between a standard quantum Hall system and this quasi 3D WPQW system.",9707188v1 1997-10-28,Investigation of acceptor levels and hole scattering mechanisms in p-gallium selenide by means of transport measurements under pressure,"The effect of pressure on acceptor levels and hole scattering mechanisms in p-GaSe is investigated through Hall effect and resistivity measurements under quasi-hydrostatic conditions up to 4 GPa. The pressure dependence of the hole concentration is interpreted through a carrier statistics equation with a single (nitrogen) or double (tin) acceptor whose ionization energies decrease under pressure due to the dielectric constant increase. The pressure effect on the hole mobility is also accounted for by considering the pressure dependencies of both the phonon frequencies and the hole-phonon coupling constants involved in the scattering rates.",9710296v1 1998-12-24,Electron Correlations in Molecular Systems,"A short review of correlated electrons in molecular systems has been performed. Main attention has been focussed on ET salts, which are the d=2 systems. They show the Mott transition in high temperatures and the transition from the antiferromagnetic to the superconducting phase in low temperatures, under a (chemical) pressure. Physical properties (the electrical resistivity, the specific heat, the magnetic susceptibility, the photoemission spectra, the optical conductivity) of ET salts have been compared with those ones in other strongly correlated systems. The optical conductivity is described in the framework of the Hubbard model, with a low frequency peak as an evidence for the Abrikosov-Suhl resonance.",9812392v1 1998-12-30,Giant transverse magnetoresistance in an asymmetric system of three GaAs/AlGaAs quantum wells in a strong magnetic field at room temperature,"The giant transverse magnetoresistance is observed in the case of photoinduced nonequilibrium carriers in an asymmetric undoped system of three GaAs/AlGaAs quantum wells at room temperature. In a magnetic field of 75 kOe, the resistance of nanostructure being studied increases by a factor of 1.85. The magnetoresistance depends quadratically on the magnetic field in low fields and tends to saturation in high fields. This phenomenon is attributed to the rearrangement of the electron wave function in magnetic field. Using the fact that the incoherent part of the scattering probability for electron scattering on impurities and bulk defects is proportional to the integral of the forth power of the envelope wave function, the calculated field dependence of the magnetoresistance is shown to be similar to that observed experimentally.",9812426v1 1999-03-03,Non linear flux flow in TiN superconducting thin film,"We have studied the superconducting behavior of 100 nm Titanium Nitride (TiN) thin film in a perpendicular magnetic field. We found a zero field transition temperature of 4.6 K and a slope in the H-T plane of -0.745 T/K. At 4.2 K, we have performed careful transport measurements by measuring both the differential resistivity and voltage as a function of a DC current. Our results are analyzed in the framework of linear and non linear flux flow behavior. In particular, we have observed an electronic instability at high vortex velocities and from its dependence with respect to the applied magnetic field, we can exctract the inelastic scattering time and diffusion length of the quasiparticles.",9903060v2 1999-08-26,Destruction of the Mott Insulating Ground State of Ca_2RuO_4 by a Structural Transition,"We report a first-order phase transition at T_M=357 K in single crystal Ca_2RuO_4, an isomorph to the superconductor Sr_2RuO_4. The discontinuous decrease in electrical resistivity signals the near destruction of the Mott insulating phase and is triggered by a structural transition from the low temperature orthorhombic to a high temperature tetragonal phase. The magnetic susceptibility, which is temperature dependent but not Curie-like decreases abruptly at TM and becomes less temperature dependent. Unlike most insulator to metal transitions, the system is not magnetically ordered in either phase, though the Mott insulator phase is antiferromagnetic below T_N=110 K.",9908390v1 1999-08-29,Anomalous microwave response of high-temperature superconducting thin-film microstrip resonator in weak dc magnetic fields,"We have studied an anomalous microwave (mw) response of superconducting YBa_{2}Cu_{3}O_{7-delta} (YBCO) microstrip resonators in the presence of a weak dc magnetic field, H_{dc}. The surface resistance (R_{s}) and reactance (X_{s}) show a correlated non-monotonic behaviour as a function of H_{dc}. R_{s} and X_{s} were found to initially decrease with elevated H_{dc} and then increase after H_{dc} reaches a crossover field, H_{c}, which is independent of the amplitude and frequency of the input mw signal within the measurements. The frequency dependence of R_{s} is almost linear at fixed H_{dc} with different magnitudes (H_{c}). The impedance plane analysis demonstrates that r_{H}, which is defined as the ratio of the change in R_{s}(H_{dc}) and that in X_{s}(H_{dc}), is about 0.6 at H_{dc}H_{c}. The H_{dc} dependence of the surface impedance is qualitatively independent of the orientation of H_{dc}.",9908429v1 2000-05-11,Magnetic Field resulting from non-linear electrical transport in single crystals of charge-ordered Pr$_{0.63}$ Ca$_{0.37}$ MnO$_{3}$},"In this letter we report that the current induced destabilization of the charge ordered (CO) state in a rare-earth manganite gives rise to regions with ferromagnetic correlation. We did this experiment by measurement of the I-V curves in single crystal of the CO system Pr$_{0.63}$Ca$_{0.37}$MnO$_{3}$ and simultanously measuring the magnetization of the current carrying conductor using a high T$_c$ SQUID working at T = 77K. We have found that the current induced destabilization of the CO state leads to a regime of negative differential resistance which leads to a small enhancement of the magnetization of the sample, indicating ferromagnetically aligned moments.",0005194v1 2000-06-22,High field magnetotransport in composite conductors: the effective medium approximation revisited,"The self consistent effective medium approximation (SEMA) is used to study three-dimensional random conducting composites under the influence of a strong magnetic field {\bf B}, in the case where all constituents exhibit isotropic response. Asymptotic analysis is used to obtain almost closed form results for the strong field magnetoresistance and Hall resistance in various types of two- and three-constituent isotropic mixtures for the entire range of compositions. Numerical solutions of the SEMA equations are also obtained, in some cases, and compared with those results. In two-constituent free-electron-metal/perfect-insulator mixtures, the magnetoresistance is asymptotically proportional to $|{\bf B}|$ at {\em all concentrations above the percolation threshold}. In three-constituent metal/insulator/superconductor mixtures a line of critical points is found, where the strong field magnetoresistance switches abruptly from saturating to non-saturating dependence on $|{\bf B}|$, at a certain value of the insulator-to-superconductor concentration ratio. This transition appears to be related to the phenomenon of anisotropic percolation.",0006351v1 2000-08-02,The Zeno effect and an inter-layer pairing mechanism for high-temperature superconductivity in layered materials,"Quantum Zeno Effect (QZE) is the suppression of the inter-subspace transition by a relatively fast intra-subspace decoherence. Earlier, we had proposed a QZE-based mechanism for the temperature-dependent normal-state c-axis resistivity of the layered high-T$_c$ cuprate superconductors in which the single-particle inter-layer tunneling is blocked by the strong intra-layer decoherence (entanglement). We now argue that while the single-particle inter-layer tunneling is thus blocked, the tunneling of the bosonic BCS-like pairs must remain unblocked inasmuch as a BCS pairing condensate is an eigenstate of the pair annihilation operator. This pair tunneling stabilizes",0008023v1 2000-12-14,Electronic Transmission Through Metallic Nanowires: Generalized Scattering Matrix Approach,"An easy to implement and powerful method for the solution of 3D scattering problems that can be well described by Helmholtz equation is presented. The matrix algebra used provides excellent stability versus the number of junctions as well as great computational speed. The matrix truncation method yields an easy single-parameter convergence procedure. Subsequently, some aspects of the electronic transport through metal nanowires are studied by the use of Landauer's scattering approach to the conductance. We predict the existence of current vortex-rings patterns due to sharp enough narrow-wide connections in atomic size point contacts. Longitudinal resonances between scattering centers provide a simple physical picture for the understanding of negative differential resistance in ideal monoatomic contacts. Relatively long nanowires with high geometrical perfection -like those recently observed by Transmission Electron Microscopy- are modelled exhibiting resonant tunnelling and total reflection at given incident energy intervals.",0012250v1 2001-03-16,Giant Magnetoresistance by Exchange Springs in DyFe$_2$/YFe$_2$ Superlattices,"Magnetization and magnetoresistance measurements are reported for antiferromagnetically coupled DyFe$_2$/YFe$_2$ multilayers in fields up to 23 T. We demonstrate that the formation of short exchange springs (~ 2 nm) in the magnetically soft YFe$_2$ layers results in a giant magneto-resistance as high as 32% in the spring region. It is shown that both the magnitude of the effect, and its dependence on magnetic field, are in good agreement with the theory of Levy and Zhang for giant magnetoresistance due to domain wall like structures.",0103354v1 2001-04-05,Fractal Nature and Scaling Exponent of Non-Drude Currents in Non-Fermi Liquids,"In many oxides of the perovskite and pseudoperovskite families there are phase transitions between insulating and normal metallic (Fermi liquid) phases that are separated by an intermediate phase that is often called a non-Fermi liquid (NFL). The dc resistivity of the intermediate or NFL phase often exhibits a T temperature dependence, in contrast to the T2 dependence expected from a bad normal metal. The same alloys exhibit a non-Drude (ND) w2alpha frequency dependence, with alpha ~ 0.5, in contrast to the Drude dependence w2 characteristic of samples with the T2 behavior. Various attempts have been made to modify the algebra of continuum Fermi liquid theory (FLT) to derive the ND exponent alpha, but these have been based on artifices designed to explain only this one parameter. The discrete filamentary model has been used to calculate many properties of high temperature superconductors, and to explain the asymmetric nature of the intermediate phase. Here it is used to derive a by the same rules previously used for several other discrete relaxation calculations that are in excellent agreement with other quite different experiments. The results are: (cubic) perovskites, alpha = 0.45, and planar conductivity of bilayered pseudoperovskites, alpha = 0.70. The corresponding experimental values are (0.4, 0.5) and 0.7.",0104095v1 2001-04-06,Evidence for high inter-granular current flow in single-phase polycrystalline MgB2 superconductor,"The distribution of magnetic field in single-phase polycrystalline bulk MgB2 has been measured using a Magneto-Optical (MO) technique for an external magnetic field applied perpendicular to the sample surface. The MO studies indicate that an inter-granular current network is readily established in this material and the current is not limited by weak-linked grain boundaries. The grain boundaries are observed to resist preferential magnetic field penetration, with the inter-grain mechanism dominating the current flow in the sample at temperatures up to 30K. The results provide clear evidence that the intra-granular current flow is isotropic. A critical current density of ~10^4 Acm-2 was estimated at 30K in a field of 150mT from the MO measurements. These results provide further evidence of the considerable potential for MgB2 for engineering applications.",0104114v1 2002-04-17,Epitaxial Growth of La$_{1/3}$Sr$_{2/3}$FeO$_3$ thin films by laser ablation,"We report on the synthesis of high quality La$_{1/3}$Sr$_{2/3}$FeO$_3$ (LSFO) thin films using the pulsed laser deposition technique on both SrTiO$_3$ (STO) and LaAlO$_3$ (LAO) substrates (100)-oriented. From X-Ray diffraction (XRD) studies, we find that the films have an out-of-plane lattice parameter around 0.3865nm, almost independent of the substrate (i.e. the nature of the strains). The transport properties reveal that, while LSFO films deposited on STO exhibit an anomaly in the resistivity vs temperature at 180K (corresponding to the charge-ordered transition and associated with a transition from a paramagnetic to an antiferromagnetic state), the films grown on LAO display a very small magnetoresistance behavior and present an hysteresis around 270K under the application of a 4T magnetic field. The changes in transport properties between both substrates are discussed and compared with the corresponding single crystals.",0204370v1 2002-05-24,The Hall effect and hole densities in high Tc GaMnAs thin films,"By studying the Hall effect in a series of low resistivity Ga1-xMnxAs samples, accurate values for the hole density p, Mn concentration x, and Curie temperature Tc are obtained over the range 0.015=1$ T) $\rho_{ff}(B)$ dependence is well fitted by the theoretical formula for that limit. That allows us to independently extract from the experimental data the values of $\sigma_{c}$ and of the ratio $\sigma _{ab}/(\sigma_{c}\gamma ^{4})$. The extracted temperature dependence $\sigma _{ab}(T)$ is consistent with microwave data. The shape of the current-voltage characteristics is also sensitive to the frequency dependence of $\sigma_{ab}$ and that allows us to estimate the quasiparticle relaxation time and relate it to the impurity bandwidth using data obtained for the same crystal.",0307450v1 2003-09-02,The enhancement of phase separation aspect in electron doped manganite Ca0.8Sm0.16Nd0.04MnO3,"The complex lanthanide doping of electron manganites results in enhancement of various phase separation effects in physical properties of these compounds. Selecting Ca0.8Sm0.16Nd0.04MnO3 as a model case we show that the first order structural phase transition from paramagnetic semi-metallic phase into anti-ferromagnetic semi-metallic phase at TS ~ 158 +- 4 K is marked by an abrupt decrease in magnetization, a step like anomaly DL/L = 10-4 in thermal expansion and large latent heat DQ = 610 J/mol. In a certain temperature range below TS, the high field magnetization exhibits hysteretic metamagnetic behavior due to field-induced first order transformation. ac-susceptibility, magnetization and resistivity data suggest rather a non-uniform state in Ca0.8Sm0.16Nd0.04MnO3 at low temperatures. The metal - insulator transition occurs at TMI ~112 +- 3 K, accompanied by a step-like increase in magnetization. These features could be ascribed to ""sponging"" of electrons from neighboring anti-ferromagnetic matrix by clusters undergoing the ferromagnetic ordering.",0309065v1 2003-12-28,Optical properties of pyrochlore oxide $Pb_{2}Ru_{2}O_{7-δ}$,"We present optical conductivity spectra for $Pb_{2}Ru_{2}O_{7-{\delta}}$ single crystal at different temperatures. Among reported pyrochlore ruthenates, this compound exhibits metallic behavior in a wide temperature range and has the least resistivity. At low frequencies, the optical spectra show typical Drude responses, but with a knee feature around 1000 \cm. Above 20000 \cm, a broad absorption feature is observed. Our analysis suggests that the low frequency responses can be understood from two Drude components arising from the partially filled Ru $t_{2g}$ bands with different plasma frequencies and scattering rates. The high frequency broad absorption may be contributed by two interband transitions: from occupied Ru $t_{2g}$ states to empty $e_{g}$ bands and from the fully filled O 2p bands to unoccupied Ru $t_{2g}$ states.",0312662v1 2004-01-31,Unprecedented Superconductivity in the beta-Pyrochlore Osmate KOs2O6,"Superconductivity in the potassium osmium oxide KOs2O6 crystallizing in the beta-pyrochlore structure is studied by means of electrical resistivity, magnetic susceptibility and specific heat. It is the second superconductor in the family of pyrochlore oxides, following the alfa-type pyrochlore oxide Cd2Re2O7 which is believed to be a conventional s-wave superconductor. The superconducting transition temperature Tc of KOs2O6 is 9.6 K, almost one order higher than the Tc = 1.0 K of Cd2Re2O7. Moreover, the superconductivity of KOs2O6 is remarkably robust under high magnetic fields, with a large upper critical magnetic field Hc2 of about 38 T, which seems to exceed Pauli's limit expected for conventional superconductivity. This is also in contrast to the case of Cd2Re2O7, in which the Hc2 is 0.29 T, much smaller than the corresponding Pauli's limit. These distinct contrasts strongly suggest that the mechanism of superconductivity is essentially different between the two pyrochlore oxides.",0402006v3 2004-03-31,Spin-Transfer Effects in Nanoscale Magnetic Tunnel Junctions,"We report measurements of magnetic switching and steady-state magnetic precession driven by spin-polarized currents in nanoscale magnetic tunnel junctions with low-resistance, < 5 Ohm-micron-squared, barriers. The current densities required for magnetic switching are similar to values for all-metallic spin-valve devices. In the tunnel junctions, spin-transfer-driven switching can occur at voltages that are high enough to quench the tunnel magnetoresistance, demonstrating that the current remains spin-polarized at these voltages.",0404002v2 2004-08-16,"Structural, transport, magnetic properties and Raman spectroscopy of orthorhombic Y$1-x$CaxMnO3(0 <= x <= 0.5)","Orthorhombic Y$_{1-x}$Ca$_x$MnO$_3$ ($0 \leq x \leq 0.5$) was prepared under high pressure and the variations with $x$ of its structural, magnetic, electrical properties and the polarized Raman spectra were investigated. The lattice parameters change systematically with $x$. Although there are strong indications for increasing disorder above $x = 0.20$, the average structure remains orthorhombic in the whole substitutional range. Ca doping increases conductivity, but temperature dependence of resistivity $\rho$(T) remains semiconducting for all $x$. The average magnetic exchange interaction changes from antiferromagnetic for $x < 0.08$ to ferromagnetic for $x > 0.08$. The evolution with $x$ of the Raman spectra provides evidence for increasingly disordered oxygen sublattice at $x \geq 0.10$, presumably due to quasistatic and/or dynamical Jahn-Teller distortions.",0408360v1 2004-09-08,Evidence for charge Kondo effect in superconducting Tl-doped PbTe,"We report results of low-temperature thermodynamic and transport measurements of Pb_{1-x}Tl_{x}Te single crystals for Tl concentrations up to the solubility limit of approximately x = 1.5%. For all doped samples, we observe a low-temperature resistivity upturn that scales in magnitude with the Tl concentration. The temperature and field dependence of this upturn are consistent with a charge Kondo effect involving degenerate Tl valence states differing by two electrons, with a characteristic Kondo temperature T_K ~ 6 K. The observation of such an effect supports an electronic pairing mechanism for superconductivity in this material and may account for the anomalously high T_c values.",0409174v2 2004-09-08,Tailoring of ferromagnetic Pr0.85Ca0.15MnO3/ferroelectric Ba0.6Sr0.4TiO3 superlattices for multiferroic properties,"Superlattices composed of ferromagnetic Pr0.85Ca0.15MnO3 and ferroelectric Ba0.6Sr0.4TiO3 layers were fabricated on (100) SrTiO3 substrates by a pulsed-laser deposition method. The capacitance and resistive parts of the samples were analyzed from the complex impedance measurements, performed on the samples using a special experimental set-up. The superlattice with larger ferroelectric thickness shows unique characteristics which are not present in the parent ferromagnetic thin film. The superlattice show both ferromagnetic and ferroelectric transitions which is an evidence for the coexistence of both the properties. The high magnetoresistance (40 % at 80K) shown by the superlattice can be attributed to the coupling between ferromagnetic and ferroelectric layers, i.e, to the magnetoelectric effect.",0409182v1 2004-09-20,Effect of Joule heating in current-driven domain wall motion,"It was found that high current density needed for the current-driven domain wall motion results in the Joule heating of the sample. The sample temperature, when the current-driven domain wall motion occurred, was estimated by measuring the sample resistance during the application of a pulsed-current. The sample temperature was 750 K for the threshold current density of 6.7 x 10^11 A/m2 in a 10 nm-thick Ni81Fe19 wire with a width of 240 nm. The temperature was raised to 830 K for the current density of 7.5 x 10^11 A/m2, which is very close to the Curie temperature of bulk Ni81Fe19. When the current density exceeded 7.5 x 10^11 A/m2, an appearance of a multi-domain structure in the wire was observed by magnetic force microscopy, suggesting that the sample temperature exceeded the Curie temperature.",0409494v1 2004-11-12,Observation of abrupt first-order metal-insulator transition in GaAs-based two-terminal device,"An abrupt first-order metal-insulator transition (MIT) as a jump of the density of states is observed for Be doped GaAs, which is known as a semiconductor, by inducing very low holes of approximately n_p=5x10^{14} cm^{-3} into the valence band by the electric field; this is anomalous. In a higher hole doping concentration of n_p=6x10^{16} cm^{-3}, the abrupt MIT is not observed at room temperature, but measured at low temperature. A large discontinuous decrease of photoluminescence intensity at 1.43 eV energy gap and a negative differential resistance are also observed as further evidence of the MIT. The abrupt MIT does not undergo a structural phase transition and is accompanied with inhomogeneity. The upper limit of the temperature allowing the MIT is deduced to be approximately 440K from experimental data. The abrupt MIT rather than the continuous MIT is intrinsic and can explain the ""breakdown"" phenomenon (unsolved problem) incurred by a high electric field in semiconductor devices.",0411328v2 2004-11-13,Large magnetoresistance anomalies in Dy7Rh3,"The compound Dy7Rh3 ordering antiferromagnetically below (TN=) 59 K has been known to exhibit a temperature (T) dependent electrical resistivity (rho) behavior in the paramagnetic state unusual for intermetallic compounds in the sense that there is a broad peak in rho(T) in the paramagnetic state (around 130 K) as though there is a semi-conductor to metal transition. In addition, there is an upturn below T_N due to magnetic super-zone gap effects. Here we report the influence of external magnetic field (H) on the rho(T) behavior of this compound below 300 K. The rise of rho(T) found below TN could be suppressed at very high fields (>> 60 kOe), thus resulting in a very large magnetoresistance (MR) in the magnetically ordered state. The most notable finding is that the magnitude of MR is large for moderate applications of H (say 80 kOe) in a temperature range far above T_N as well, which is untypical of intermetallic compounds. Thus, this compound is characterized by large MR anomalies in the entire T range of investigation.",0411360v1 2004-11-24,"Large magnetoresistance in the magnetically ordered state as well as in the paramagnetic state near 300 K in an intermetallic compound,Gd7Rh3","We report the response of electrical resistivity $\rho$ to the application of magnetic fields (H) up to 140 kOe in the temperature interval 1.8-300 K for the compound, Gd7Rh3, ordering antiferromagnetically below 150 K. We find that there is an unusually large decrease of $\rho$ for moderate values of H in the close vicinity of room temperature uncharacteristic of paramagnets, with the magnitude of the magnetoresistance increasing with decreasing temperature as though the spin-order contribution to $\rho$ is temperature dependent. In addition, this compound exhibits giant magnetoresistance behaviour at rather high temperatures (above 77 K) in the magnetically ordered state due to a metamagnetic transition.",0411608v1 2005-04-05,Coherent transport in homojunction between excitonic insulator and semimetal,"From the solution of a two-band model, we predict that the thermal and electrical transport across the junction of a semimetal and an excitonic insulator will exhibit high resistance behavior and low entropy production at low temperatures, distinct from a junction of a semimetal and a normal semiconductor. This phenomenon, ascribed to the dissipationless exciton flow which dominates over the charge transport, is based on the much longer length scale of the change of the effective interface potential for electron scattering due to the coherence of the condensate than in the normal state.",0504121v1 2005-04-25,Impurity scattering and quantum confinement in giant magnetoresistance systems,"Ab initio calculations for the giant magnetoresistance (GMR) in Co/Cu, Fe/Cr, and Fe/Au multilayers are presented. The electronic structure of the multilayers and the scattering potentials of point defects therein are calculated self-consistently. Residual resistivities are obtained by solving the quasi-classical Boltzmann equation including the electronic structure of the layered system, the anisotropic scattering cross sections derived by a Green's function method and the vertex corrections. Furthermore, the influence of scattering centers at the interfaces and within the metallic layers is incorporated by averaging the scattering cross sections of different impurities at various sites. An excellent agreement of experimental and theoretical results concerning the general trend of GMR in Co/Cu systems depending on the type and the position of impurities is obtained. Due to the quantum confinement in magnetic multilayers GMR can be tailored as a function of the impurity position. In Co/Cu and Fe/Au systems impurities in the magnetic layer lead to high GMR values, whereas in Fe/Cr systems defects at the interfaces are most efficient to increase GMR.",0504634v1 2005-05-16,Novel procedure to prepare cadmium stannate films using spray pyrolysis technique for solar cell applications,"Thin films of cadmium stannate was prepared using low cost cadmium acetate and tin (II) chloride precursors by spray pyrolysis technique at three different substrate temperatures of 400, 450 and 5000 C. A novel procedure of simultaneously forming additional layer, introduced for the first time in this work, on the already coated cadmium stannate film reduced the sheet resistance from 160 ohms/sq to 15 ohms/sq. Further, it is identified that the formation of additional layer does not affect the structural and optical properties of the cadmium stannate films, but improves the electrical property; thus the formation of additional layer seems to be an effective alternate for annealing the films at high temperature in the presence of Ar, CdS, Ar/CdS mixture, hydrogen or nitrogen to improve the structural, electrical and optical properties of the cadmium stannate films as has been reported in the literature. The maximum optical transmittance value of the prepared cadmium stannate film is about 99.8 % and the optical band gap energy value is about 2.9 eV.",0505383v1 2005-05-30,Mechanisms limiting the coherence time of spontaneous magnetic oscillations driven by DC spin-polarized currents,"The spin-transfer torque from a DC spin-polarized current can generate highly-coherent magnetic precession in nanoscale magnetic-multilayer devices. By measuring linewidths of spectra from the resulting resistance oscillations, we argue that the coherence time can be limited at low temperature by thermal deflections about the equilibrium magnetic trajectory, and at high temperature by thermally-activated transitions between dynamical modes. Surprisingly, the coherence time can be longer than predicted by simple macrospin simulations.",0505733v2 2005-06-05,On the unusual behavior of nitride compounds,"This report presents consistent insight into the mechanism behind the unusual behavior of nitride compounds from the perspective of tetrahedron bond formation and its consequence on valence density of states. An extension of the recent bond-band-barrier (BBB) correlation mechanism for oxidation [Sun CQ, Prog Mater Sci 2003;48:521-685] to the electronic process of nitridation has led to the essentiality of sp-orbital hybridization for a nitrogen atom upon interacting with atoms in solid phase of arbitrary less-electronegative element. In the process of nitridation, a nitrogen atom forms a quasi-tetrahedron with surrounding host atoms through bonding and nonbonding interaction associated with production of electronic holes and antibonding dipoles, which add corresponding density of states to the valence band of the host. It is suggested that the valance alteration of the system takes the responsibility for the blue shift in photoluminescence, lowered work function for cold cathode field emission, corrosion and wear resistant, high elasticity, and magnetic modulation as well.",0506109v1 2005-06-10,"Anisotropic Magnetoresistance and Magnetic Anisotropy in High-quality (Ga,Mn)As Films","We have performed a systematic investigation of magnetotransport of a series of as-grown and annealed Ga1-xMnxAs samples with 0.011 <= x <= 0.09. We find that the anisotropic magnetoresistance (AMR) generally decreases with increasing magnetic anisotropy, with increasing Mn concentration and on low temperature annealing. We show that the uniaxial magnetic anisotropy can be clearly observed from AMR for the samples with x >= 0.02. This becomes the dominant anisotropy at elevated temperatures, and is shown to rotate by 90o on annealing. We find that the in-plane longitudinal resistivity depends not only on the relative angle between magnetization and current direction, but also on the relative angle between magnetization and the main crystalline axes. The latter term becomes much smaller after low temperature annealing. The planar Hall effect is in good agreement with the measured AMR indicating the sample is approximately in a single domain state throughout most of the magnetisation reversal, with a two-step magnetisation jump ascribed to domain wall nucleation and propagation.",0506250v1 2005-06-14,The O-M-O triatomic molecule: Basic unit of cuprates & manganates,"The O(oxygen)-M(metal)-O(oxygen) molecule is a basic unit of high-temperature superconducting cuprates and colossal magnetoresistance exhibiting manganates. This molecule can be regarded either as an element of a linear chain or as an ingredient of the corresponding cuprate or manganate lattice. The symmetry of the unit being different in the two approaches, group theory imposes different limitations on conceivable vibrational modes and atomic otbitals that control its transport and optical properties. We now calculate the electron hopping energies along Cu(P0-O(A) bonds, sites for nonlocal electron-vibrational mode coupling. We find the electric transport along the O(A)-Cu(P)-O(A) molecule dominated by scattering from bond polarons which is reflected in the two-branch character of the temperature dependence of its electric resistance.",0506308v1 2005-09-27,Critical currents and vortex dynamics in percolative superconductors containing fractal clusters of a normal phase,"The effect of fractal clusters on magnetic and transport properties of percolative superconductors is considered. The superconductor contains percolative superconducting cluster, carrying a transport current, as well as clusters of a normal phase, which act as pinning centers. A prototype of such a structure is a high-temperature superconducting wire. It is found that normal-phase clusters can have fractal features that affect the vortex dynamics. The fractal dimension of the normal-phase cluster boundary in YBCO films is estimated. Depinning and transport of vortices in fractal superconducting structures are investigated. The current-voltage characteristics of superconductors containing fractal clusters are obtained. Dependencies of free vortex density on the fractal dimension as well as the resistance on the transport current are studied. It is found that the fractality of the cluster boundary intensifies pinning. This feature enables the current-carrying capability of a superconductor to be enhanced without changing of its chemical composition.",0509701v1 2005-10-18,Surface Roughness and Hydrodynamic Boundary Conditions,"We report results of investigations of a high-speed drainage of thin aqueous films squeezed between randomly nanorough surfaces. A significant decrease in hydrodynamic resistance force as compared with predicted by Taylor's equation is observed. However, this reduction in force does not represents the slippage. The measured force is exactly the same as that between equivalent smooth surfaces obeying no-slip boundary conditions, but located at the intermediate position between peaks and valleys of asperities. The shift in hydrodynamic thickness is shown to be independent on the separation and/or shear rate. Our results disagree with previous literature data reporting very large and shear-dependent boundary slip for similar systems.",0510462v2 2005-10-20,Current-driven magnetization switching in CoFeB/MgO/CoFeB magnetic tunnel junctions,"Current-driven magnetization switching in low-resistance Co40Fe40B20/MgO/Co40Fe40B20 magnetic tunnel junctions (MTJs) is reported. The critical-current densities Jc required for current-driven switching in samples annealed at 270C and 300C are found to be as low as 7.8 x 10^5 A/cm^2 and 8.8 x 10^5 A/cm^2 with accompanying tunnel magnetoresistance (TMR) ratios of 49% and 73 %, respectively. Further annealing of the samples at 350C increases TMR ratio to 160 %, while accompanying Jc increases to 2.5 x 10^6 A/cm^2. We attribute the low Jc to the high spin-polarization of tunnel current and small MsV product of the CoFeB single free layer, where Ms is the saturation magnetization and V the volume of the free layer.",0510538v1 2006-02-13,Doping of Ce in T-La2CuO4: Rigorous test for electron-hole symmetry for high-Tc superconductivity,"We report that Ce doping was achieved in La2CuO4 with the K2NiF4 (T) structure for the first time by molecular beam epitaxy. A synthesis temperature of as low as ~ 630C and an appropriate substrate choice, i.e., (001)LaSrGaO4 (a \~ 3.843 A), enebled us to incorporate Ce into K2NiF4 lattice and to obtain Ce-doped T-La2-xCexCuO4 up to x ~ 0.06. The doping of Ce makes T-La2CuO4 more insulating, which is in sharp contrast to Sr (or Ba) doping in T-La2CuO4, which make the compound metallic and superconducting. The observed smooth increase in resistivity from the hole-doped side (T-La2-xSrxCuO4) to the electron-doped side (T-La2-xCexCuO4) indicates that the electron-hole symmetry is broken in the T-phase materials.",0602303v1 2006-03-02,Coupled dynamics of electrons and phonons in metallic nanotubes: current saturation from hot phonons generation,"We show that the self-consistent dynamics of both phonons and electrons is the necessary ingredient for the reliable description of the hot phonons generation during electron transport in metallic single-wall carbon nanotubes (SWNTs). We solve the coupled Boltzmann transport equations to determine in a consistent way the current vs. voltage (IV) curve and the phonon occupation in metallic SWNTs which are lying on a substrate. We find a good agreement with measured IV curves and we determine an optical phonon occupation which corresponds to an effective temperature of several thousands K (hot phonons), for the voltages typically used in experiments. We show that the high-bias resistivity strongly depends on the optical phonon thermalization time. This implies that a drastic improvement of metallic nanotubes performances can be achieved by increasing the coupling of the optical phonons with a thermalization source.",0603046v1 2006-03-05,Electro-Thermal Transport in Metallic Single-Wall Carbon Nanotubes for Interconnect Applications,"This work represents the first electro-thermal study of metallic single-wall carbon nanotubes (SWNTs) for interconnect applications. Experimental data and careful modeling reveal that self-heating is of significance in short (1 < L < 10 um) nanotubes under high-bias. The low-bias resistance of micron scale SWNTs is also found to be affected by optical phonon absorption (a scattering mechanism previously neglected) above 250 K. We also explore length-dependent electrical breakdown of SWNTs in ambient air. Significant self-heating in SWNT interconnects can be avoided if power densities per unit length are limited to less than 5 uW/um.",0603110v1 2006-03-24,Single-crystalline nanopillars for spin-transfer measurements,"We report on current-induced magnetization switching (CIMS) in single- crystalline nanopillars. Fe(14 nm)/Cr(0.9 nm)/Fe(10 nm)/Ag(6 nm)/Fe(2 nm) multilayers are deposited by molecular-beam epitaxy. The central Fe layer is coupled to the thick one by interlayer exchange coupling over Cr. The topmost Fe layer is decoupled (free layer). Nanopillars with 150 nm diameter are prepared by optical and e-beam lithography. The opposite spin scattering asymmetries of Fe/Cr and Fe/Ag interfaces enable us to observe CIMS at small magnetic fields and opposite current polarity in a single device. At high magnetic fields, step-like resistance changes are measured at positive currents and are attributed to current-driven magnetic excitations.",0603662v1 2006-07-03,Knight shift detection using gate-induced decoupling of the hyperfine interaction in quantum Hall edge channels,"A method for the observation of the Knight shift in nanometer-scale region in semiconductors is developed using resistively detected nuclear magnetic resonance (RDNMR) technique in quantum Hall edge channels. Using a gate-induced decoupling of the hyperfine interaction between electron and nuclear spins, we obtain the RDNMR spectra with or without the electron-nuclear spin coupling. By a comparison of these two spectra, the values of the Knight shift can be given for the nuclear spins polarized dynamically in the region between the relevant edge channels in a single two-dimensional electron system, indicating that this method has a very high sensitivity compared to a conventional NMR technique.",0607028v1 2006-12-01,New Type Phase Transition of Li2RuO3 with Honeycomb Structure,"A new-type structural transition has been found in Li2RuO3 with honeycomb lattice of edge-sharing RuO6-octahedra. With decreasing temperature T, the electrical resistivity exhibits an anomalous increase at T=Tc~540 K, suggesting the (metal to insulator)-like transition and the magnetic susceptibility also shows a sharp decrease. Detailed structure analyses have revealed that the high temperature space group C2/m changes to P21/m at Tc. The most striking fact is that a significant reduction of the bond lengths is found between two of six Ru-Ru pairs of the hexagon in the low temperature phase, indicating a new type phase transition by the mechanism of the formation of molecular orbits of these Ru-Ru pairs.",0612026v1 2006-12-26,Transport properties of n-type ultrananocrystalline diamond films,"We investigate transport properties of ultrananocrystalline diamond films for a broad range of temperatures. Addition of nitrogen during plasma-assisted growth increases the conductivity of ultrananocrystalline diamond films by several orders of magnitude. We show that films produced at low concentration of nitrogen in the plasma are very resistive and electron transport occurs via a variable range hopping mechanism while in films produced at high nitrogen concentration the electron states become delocalized and the transport properties of ultrananocrystalline diamond films can be described using the Boltzmann formalism. We discuss the critical concentration of carriers at which the metal to insulator transition in ultrananocrystalline diamond films occurs and compare our results with available experimental data.",0612633v1 2007-01-29,Parameters of the Dzyaloshinsky-Moriya type weak ferromagnetism for some perovskite compounds,"Compounds with distorted perovskite structure of the 4-f and 3-d transition metals with the common formula LnTO3 (where Ln is rare-earth element, T is an element from the Fe group) are the most multifold binary oxides of these two groups elements. Wide range of stability for this structure allows the realization of combinations of the Lanthanides with all the transition metals except the Nickel. Quite interesting physical phenomena take place in these oxides like charge and orbital ordering; relatively independent magnetic lattices of the both metals; particular magnetic structures; high optical indicators; giant magneto-resistance; peculiar dielectric and ferroelectric properties etc. We have investigated the magnetic properties of pure ferrites and chromium-based materials as well as of some mixed type oxides like HoxTb1-xO3, HoMnxFe1-xO3, HoMnxCr1-xO3 and DyFexCr1-xO3.",0701708v1 2007-02-20,Organic small molecule field-effect transistors with Cytop(TM) gate dielectric: eliminating gate bias stress effects,"We report on organic field-effect transistors with unprecedented resistance against gate bias stress. The single crystal and thin-film transistors employ the organic gate dielectric Cytop(TM). This fluoropolymer is highly water repellent and shows a remarkable electrical breakdown strength. The single crystal transistors are consistently of very high electrical quality: near zero onset, very steep subthreshold swing (average: 1.3 nF V/(dec cm2)) and negligible current hysteresis. Furthermore, extended gate bias stress only leads to marginal changes in the transfer characteristics. It appears that there is no conceptual limitation for the stability of organic semiconductors in contrast to hydrogenated amorphous silicon.",0702472v1 2007-02-25,Broadband dielectric microwave microscopy on $μ$m length scales,"We demonstrate that a near-field microwave microscope based on a transmission line resonator allows imaging in a substantially wide range of frequencies, so that the microscope properties approach those of a spatially-resolved impedance analyzer. In the case of an electric probe, the broadband imaging can be used in a direct fashion to separate contributions from capacitive and resistive properties of a sample at length scales on the order of one micron. Using a microwave near-field microscope based on a transmission line resonator we imaged the local dielectric properties of a Focused Ion Beam (FIB) milled structure on a high-dielectric-constant Ba_{0.6}Sr_{0.4}TiO_3 (BSTO) thin film in the frequency range from 1.3 GHz to 17.4 GHz. The electrostatic approximation breaks down already at frequencies above ~10 GHz for the probe geometry used, and a full-wave analysis is necessary to obtain qualitative information from the images.",0702573v1 2007-06-05,Structure-Property Relationship in the Ordered-Perovskite- Related Oxide Sr3.12Er0.88Co4O10.5,"Synchrotron X-ray diffraction patterns were measured and analyzed for a polycrystalline sample of the room-temperature ferromagnet Sr3.12Er0.88Co4O10.5 from 300 to 650 K, from which two structural phase transitions were found to occur successively. The higher-temperature transition at 509 K is driven by ordering of the oxygen vacancies, which is closely related to the metallic state at high temperatures. The lower-temperature transition at 360 K is of first order, at which the ferromagnetic state suddenly appears with exhibiting a jump in magnetization and resistivity. Based on the refined structure, possible spin and orbital models for the magnetic order are proposed.",0706.0605v2 2007-08-14,Origin of the Non-Linear Pressure Effects in Perovskite Manganites: Buckling of Mn-O-Mn Bonds and Jahn-Teller Distortion of the MnO6 Octahedra Induced by Pressure,"High-pressure resistivity and x-ray diffraction have been measured on La0.85MnO3-d. At low pressures the metal-insulator transition temperature (TMI) increases linearly with pressure up to a critical pressure, P* ~ 3.4 GPa, which is followed by reduction of TMI with increasing pressure. Analysis of the bond distances and bond angles reveal that a bandwidth increase drives the in-crease of TMI for pressure below P*. The reduction of TMI at higher pressures is found to result from Jahn-Teller distortions of the MnO6 octahedra. The role of anharmonic interatomic potential is discussed.",0708.1963v2 2007-08-15,Insulator to semiconductor transition and magnetic properties of the one-dimensional S = 1/2 system In_2VO_5,"We report structural, magnetization, electrical resistivity and nuclear- and electron spin resonance data of the complex transition metal oxide In_2VO_5 in which structurally well-defined V-O chains are realized. An itinerant character of the vanadium d-electrons and ferromagnetic correlations, revealed at high temperatures, are contrasted with the insulating behavior and predominantly antiferromagnetic exchange between the localized V^{4+} S = 1/2-magnetic moments which develop below a certain characteristic temperature T* ~ 120 K. Eventually the compound exhibits short-range magnetic order at $T_SRO ~ 20 K. We attribute this crossover occurring around T* to the unusual anisotropic thermal contraction of the lattice which changes significantly the overlap integrals and the character of magnetic intra- and interchain interactions.",0708.2088v1 2007-11-15,Recrystallization of glass: homogeneous vs. heterogeneous nucleation in La(0.5)Ca(0.5)MnO3,"We probe through magnetization and resistivity measurements a kinetically arrested glass-like but long-range ordered magnetic state. The transformation kinetics of the magnetic field-temperature induced broad first-order transition from ferromagnetic-metallic (FMM) to antiferromagnetic-insulating (AFI) state gets hindered at low temperature in a La(0.5)Ca(0.5)MnO3 sample. A fraction of high-temperature FMM phase persists to the lowest temperature, albeit as a non-ergodic state. We present a phenomenology for this glass-like but long-range order FMM phase which devitrifies on heating and converts to equilibrium AFI phase. The residual kinetically arrested FMM phase can be `recrystallized' to AFI state by annealing and more efficiently by successive annealing, presumably by heterogeneous nucleation. This glass-like state shows a stimulating feature that when the fraction of glass is larger the `recrystallization' is easier.",0711.2347v1 2007-11-28,Radiation Damage in Polarized Ammonia Solids,"Solid NH3 and ND3 provide a highly polarizable, radiation resistant source of polarized protons and deuterons and have been used extensively in high luminosity experiments investigating the spin structure of the nucleon. Over the past twenty years, the UVA polarized target group has been instrumental in producing and polarizing much of the material used in these studies, and many practical considerations have been learned in this time. In this discussion, we analyze the polarization performance of the solid ammonia targets used during the recent JLab Eg4 run. Topics include the rate of polarization decay with accumulated charge, the annealing procedure for radiation damaged targets to recover polarization, and the radiation induced change in optimum microwave frequency used to polarize the sample. We also discuss the success we have had in implementing frequency modulation of the polarizing microwave frequency.",0711.4413v1 2008-03-06,Field emission from single multi-wall carbon nanotubes,"Electron field emission characteristics of individual multiwalled carbon nanotubes have been investigated by a piezoelectric nanomanipulation system operating inside a scanning electron microscopy chamber. The experimental setup ensures a high control capability on the geometric parameters of the field emission system (CNT length, diameter and anode-cathode distance). For several multiwalled carbon nanotubes, reproducible and quite stable emission current behaviour has been obtained with a dependence on the applied voltage well described by a series resistance modified Fowler-Nordheim model. A turn-on field of about 30 V/um and a field enhancement factor of around 100 at a cathode-anode distance of the order of 1 um have been evaluated. Finally, the effect of selective electron beam irradiation on the nanotube field emission capabilities has been extensively investigated.",0803.0810v1 2008-04-10,Electronic properties and phase transitions in low-dimensional semiconductors,"We present the first review of the current state of the literature on electronic properties and phase transitions in TlX and TlMX2 (M = Ga, In; X = Se, S, Te) compounds. These chalcogenides belong to a family of the low-dimensional semiconductors possessing chain or layered structure. They are of significant interest because of their highly anisotropic properties, semi- and photoconductivity, non-linear effects in their I-V characteristics (including a region of negative differential resistance), switching and memory effects, second harmonic optical generation, relaxor behavior and potential applications for optoelectronic devices. We review the crystal structure of TlX and TlMX2 compounds, their transport properties under ambient conditions, experimental and theoretical studies of the electronic structure, transport properties and semiconductor-metal phase transitions under high pressure, and sequences of temperature-induced structural phase transitions with intermediate incommensurate states. Electronic nature of the ferroelectric phase transitions in the above-mentioned compounds, as well as relaxor behavior, nanodomains and possible occurrence of quantum dots in doped and irradiated crystals is discussed.",0804.1639v2 2008-04-23,Superconductivity at 53.5 K in GdFeAsO1-delta,"Here we report the fabrication and superconductivity of the iron-based arsenic-oxide GdFeAsO1-delta compound with oxygen-deficiency, which has an onset resistivity transition temperature at 53.5 K. This material has a same crystal structure as the newly discovered high-Tc ReFeAsO1-delta family (Re = rare earth metal) and a further reduced crystal lattice, while the Tc starts to decrease compared with the SmFeAsO1-delta system.",0804.3727v3 2008-05-28,Effect of pressure on the superconducting critical temperature of La[O_{0.89}F_{0.11}]FeAs and Ce[O_{0.88}F_{0.12}]FeAs,"We have performed several high-pressure resistivity experiments on the recently discovered superconductors La[O_{0.89}F_{0.11}]FeAs and Ce[O_{0.88}F_{0.12}]FeAs. At ambient pressure, these materials have superconducting onset temperatures T_c of 28 K and 44 K, respectively. While the T_c of La[O_{0.89}F_{0.11}]FeAs goes through a maximum between 10-68 kbar, in qualitative agreement with a recent report by Takahashi et al., the T_c of Ce[O_{0.88}F_{0.12}]FeAs decreases monotonically over the measured pressure range. At 265 kbar, the T_c of the cerium-based compound has been suppressed below 1.1 K.",0805.4372v3 2008-06-18,UV-photon and electrically driven resistance switching in ZnO nanotube arrays,"Vertically aligned ZnO nanotube arrays fabricated on an ITO substrate are found to exhibit strong persistent photoconductivity (PPC) effect and electrically driven conductance switching behavior, though the latter shows a gradual decay from high conductance state to a low conductance state. Unlike the electrical switching, the PPC cannot be reset or reversed by an electrical pulse. Excitation wavelength dependent conductance measurement indicates the presence of the defect localized states (DLS) ~ 240meV above the valence band edge, in support of the hypothesis that the doubly ionization of these DLS are responsible for the PPC effect.",0806.2907v2 2008-06-20,Ferromagnetic spin fluctuation in LaFeAsO1-xFx,"The F doped LaFeAsO, a recently discovered superconductor with the high Tc of 26 K, has been studied by the resistivity, magnetic susceptibility, and heat capacity measurements in the F doping range from 0 to 0.14 (x in LaFeAsO1-xFx). In the low temperature region, a T3lnT term in the heat capacity and a T2 term in the magnetic susceptibility, which are derived from the spin fluctuation, are observed. The nearly ferromagnetic nature evidenced by a large Wilson ratio (6.5 for x = 0, and 11.2 for x = 0.025) suggests that the superconductivity in the LaFeAsO system is mediated by ferromagnetic spin fluctuation.",0806.3304v1 2008-06-27,Magnetoresistance oscillations and relaxation effects at the SrTiO3-LaAlO3 interface,"We present low-temperature and high-field magnetotransport data on SrTiO3-LaAlO3 interfaces. The resistance shows hysteresis in magnetic field and a logarithmic relaxation as a function of time. Oscillations in the magnetoresistance are observed, showing a square root periodicity in the applied magnetic field, both in large-area unstructured samples as well as in a structured sample. An explanation in terms of a commensurability condition of edge states in a highly mobile two-dimensional electron gas between substrate step edges is suggested.",0806.4450v1 2008-07-24,Fishtail effect and the vortex phase diagram of single crystal Ba0.6K0.4Fe2As2,"By measuring the magnetization hysteresis loops of superconducting Ba0.6K0.4Fe2As2 single crystals, we obtained the high upper critical field and large current carrying ability, which point to optimistic applications. The fishtail (or second peak) effect is also found in the material, and the position of the vortex pinning force shows a maximum at 1/3 of the reduced field, being consistent with the picture of vortex pinning by small size normal cores in the sample. Together with the resistive measurements, for the first time the vortex phase diagram is obtained for superconductor Ba0.6K0.4Fe2As2.",0807.3786v3 2008-07-25,Adaptation of the Bridgman anvil cell to liquid pressure mediums,"The advantage of Bridgman anvil pressure cells is their wide pressure range and the large number of wires which can be introduced into the pressure chamber. In these pressure cells soft solid pressure mediums like steatite are used. We have succeeded in adapting the Bridgman cell to liquid pressure mediums. With this breakthrough it is now possible to measure in very good hydrostatic pressure conditions up to 7 GPa, which is about twice the pressure attainable in piston-cylinder cells. The pressure gradient in the cell, estimated from the superconducting transition width of lead, is reduced by a factor of five in the liquid medium with respect to steatite. By the use of non-magnetic materials for the anvils and the clamp and due to the small dimensions of the latter, our device is specially suitable for magneto-transport measurements in dilution fridges. This pressure cell has been developed to measure very fragile and brittle samples like organic conductors. Resistivity measurements of (TMTTF)2BF4 performed in a solid and liquid pressure medium demonstrate the necessity of hydrostatic pressure conditions for the study of organic conductors at high pressures.",0807.4137v1 2008-08-15,"Localization and the Anomalous Hall Effect in a ""Dirty"" Metallic Ferromagnet","We report magnetoresistance measurements over an extensive temperature range (0.1 K $\leq T \leq$ 100 K) in a disordered ferromagnetic semiconductor (\gma). The study focuses on a series of metallic \gma~ epilayers that lie in the vicinity of the metal-insulator transition ($k_F l_e\sim 1$). At low temperatures ($T < 4$ K), we first confirm the results of earlier studies that the longitudinal conductivity shows a $T^{1/3}$ dependence, consistent with quantum corrections from carrier localization in a ``dirty'' metal. In addition, we find that the anomalous Hall conductivity exhibits universal behavior in this temperature range, with no pronounced quantum corrections. We argue that observed scaling relationship between the low temperature longitudinal and transverse resistivity, taken in conjunction with the absence of quantum corrections to the anomalous Hall conductivity, is consistent with the side-jump mechanism for the anomalous Hall effect. In contrast, at high temperatures ($T \gtrsim 4$ K), neither the longitudinal nor the anomalous Hall conductivity exhibit universal behavior, indicating the dominance of inelastic scattering contributions down to liquid helium temperatures.",0808.2079v2 2008-08-22,Phase Coherence Effects in the Vortex Transport Entropy,"Nernst and electrical resistivity measurements in superconducting YBCO and BSCCO with and without columnar defects show a distinctive thermodynamics of the respective liquid vortex matter. At a field dependent high temperature region in the phase diagram the Nernst signal is independent of structural defects in both materials. At lower temperatures, in YBCO, defects contribute only to the vortex mobility and the transport entropy is that of a system of vortex lines. The transition to lower temperatures in BSCCO has a different origin, the maximum in the Nernst signal when decreasing temperature is not associated with transport properties but with the entropy behavior of pancake vortices in the presence of structural defects.",0808.3015v1 2009-02-05,Itinerant antiferromagnetism in BaCr$_2$As$_2$,"We report single crystal synthesis, specific heat and resistivity measurements and electronic structure calculations for BaCr$_2$As$_2$. This material is a metal with itinerant antiferromagnetism, similar to the parent phases of Fe-based high temperature superconductors, but differs in magnetic order. Comparison of bare band structure density of states and the low temperature specific heat implies a mass renormalization of $\sim$ 2. BaCr$_2$As$_2$ shows stronger transition metal - pnictogen covalency than the Fe compounds, and in this respect is more similar to BaMn$_2$As$_2$. This provides an explanation for the observation that Ni and Co doping is effective in the Fe-based superconductors, but Cr or Mn doping is not.",0902.0945v2 2009-04-05,Superconductivity in Ir-doped LaFe1-xIrxAsO,"We report the realization of superconductivity by 5d element Ir doping in LaFeAsO, a prototype parent compound of high-temperature iron based superconductors. X-ray diffraction patterns indicate that the material has formed the ZrCuSiAs-type structure with a space group P4/nmm. The systematic evolution of the lattice constants demonstrated that the Fe ions were successfully replaced by the Ir. Both electrical resistance and magnetization measurements show superconductivity up to 11 K in LaFe1-xIrxAsO. The superconducting transitions at different magnetic fields were also measured yielding a slope of -dHc2/dT = 6.7 T / K near Tc, and the upper critical field at zero K is found to be about 55 T. This is the first example of bulk superconductivity induced by replacing the Fe sites with higher d-orbital electrons in FeAs-1111 family, which should add more ingredients to the underlying physics of the iron-based superconductors.",0904.0772v4 2009-04-06,Gap opening in the zeroth Landau level of graphene,"We have measured a strong increase of the low-temperature resistivity $\rho_{xx}$ and a zero-value plateau in the Hall conductivity $\sigma_{xy}$ at the charge neutrality point in graphene subjected to high magnetic fields up to 30 T. We explain our results by a simple model involving a field dependent splitting of the lowest Landau level of the order of a few Kelvin, as extracted from activated transport measurements. The model reproduces both the increase in $\rho_{xx}$ and the anomalous $\nu=0$ plateau in $\sigma_{xy}$ in terms of coexisting electrons and holes in the same spin-split zero-energy Landau level.",0904.0948v1 2009-07-09,Agglomeration and filtration of colloidal suspensions with DVLO interactions in simulation and experiment,"Cake filtration is a widely used solid-liquid separation process. However, the high flow resistance of the nanoporous filter cake lowers the efficiency of the process significantly. The structure and thus the permeability of the filter cakes depend on the compressive load acting on the particles, the particles size, and the agglomeration of the particles. The latter is determined by the particle charge and the ionic strength of the suspension, as described by the Derjaguin-Landau-Verwey-Overbeek (DLVO) theory. In this paper, we propose a combined stochastic rotation dynamics (SRD) and molecular dynamics (MD) methodology to simulate the cake formation. The simulations give further insight into the dependency of the filter cakes' structure on the agglomeration of the particles, which cannot be accessed experimentally. The permeability, as investigated with lattice Boltzmann (LB) simulations of flow through the discretized cake, depends on the particle size and porosity, and thus on the agglomeration of the particles. Our results agree qualitatively with experimental data obtained from colloidal boehmite suspensions.",0907.1551v2 2009-07-12,Vortex-like state observed in ferromagnetic contacts,"Point-contacts (PC) offer a simple way to create high current densities, 10^9 A/cm^2 and beyond, without substantial Joule heating. We have shown recently (Nano Letters, 7 (2007) 927) that conductivity of nanosized PCs between a normal and ferromagnetic metals exhibits bi-stable hysteretic states versus both bias current and external magnetic field - the effect typical for spin-valve structures. Here we report that apart from the bi-stable state a third intermediate-resistance state is occasionally observed. We interpret this state as due to a spin-vortex in the PC, nucleated either by Oersted field of the bias current and/or by the circular geometry of PC. The observed three-level-states in the PC conductivity testify that the interface spins are both weakly coupled to the spins in the bulk and have depressed exchange interaction within the surface layer.",0907.2027v2 2009-07-16,Dynamical correlations in electronic transport through a system of coupled quantum dots,"Current auto- and cross-correlations are studied in a system of two capacitively coupled quantum dots. We are interested in a role of Coulomb interaction in dynamical correlations, which occur outside the Coulomb blockade region (for high bias). After decomposition of the current correlation functions into contributions between individual tunneling events, we can show which of them are relevant and lead to sub-/supper-Poissonian shot noise and negative/positive cross-correlations. The results are differentiated for a weak and strong inter-dot coupling. Interesting results are for the strong coupling case when electron transfer in one of the channel is strongly correlated with charge drag in the second channel. We show that cross-correlations are non-monotonic functions of bias voltage and they are in general negative (except some cases with asymmetric tunnel resistances). This is effect of local potential fluctuations correlated by Coulomb interaction, which mimics the Pauli exclusion principle.",0907.2879v1 2009-07-30,Solvothermal Reduction of Chemically Exfoliated Graphene Sheets,"Graphene has attracted much attention due to its interesting properties and potential applications. Chemical exfoliation methods have been developed to make graphene recently, aimed at large-scale assembly and applications such as composites and Li ion batteries. Although efficient, the chemical exfoliation methods involve oxidation of graphene and introduce defects in the as-made sheets. Hydrazine reduction at 100 has shown to partially restore the structure and conductance of graphite oxide. However, the reduced GO still shows strong defect peaks in Raman spectra with higher resistivity than pristine graphene by 2 to 3 orders of magnitude. It is important to produce much less defective graphene sheets than GO, and develop more effective graphene reduction. Recently, we reported a mild exfoliation-reintercalation-expansion method to form high-quality GS with higher conductivity and lower oxidation degree than GO.5 Here, we present a 180 solvothermal reduction method for our GS and GO. The solvothermal reduction is more effective than the earlier reduction methods in lowering the oxygen and defect levels in GS, increasing the graphene domains, and bringing the conductivity of GS close to pristine graphene. The reduced GS possess the highest degree of pristinity among chemically derived graphene.",0907.5417v1 2009-09-23,Intermediate-valence behavior of the transition-metal oxide CaCu$_3$Ru$_4$O$_{12}$,"The transition--metal oxide CaCu$_3$Ru$_4$O$_{12}$ with perovskite--type structure shows characteristic properties of an intermediate--valence system. The temperature--dependent susceptibility exhibits a broad maximum around $150 - 160$ K. At this temperature, neutron powder diffraction reveals a small but significant volume change whereby the crystal structure is preserved. Moreover, the temperature--dependent resistivity changes its slope. NMR Knight shift measurements of Ru reveal a cross--over from high temperature paramagnetic behavior of localized moments to itinerant band states at low temperatures. Additional density--functional theory calculations can relate the structural anomaly with the $d$--electron number. The different experimental and calculational methods result in a mutually consistent description of CaCu$_3$Ru$_4$O$_{12}$ as an intermediate--valent system in the classical sense of having low--energy charge fluctuations.",0909.4208v1 2009-10-09,Observation of a d-wave nodal liquid in highly underdoped Bi_2Sr_2CaCu_2O_{8+δ},"We use angle resolved photoemission spectroscopy to probe the electronic excitations of the non-superconducting state that exists between the antiferromagnetic Mott insulator at zero doping and the superconducting state at larger dopings in Bi_2Sr_2CaCu_2O_{8+\delta}. We find that this state is a nodal liquid whose excitation gap becomes zero only at points in momentum space. Despite exhibiting a resistivity characteristic of an insulator and the absence of coherent quasiparticle peaks, this material has the same gap structure as the d-wave superconductor. We observe a smooth evolution of the spectrum across the insulator-to-superconductor transition, which suggests that high temperature superconductivity emerges when quantum phase coherence is established in a non-superconducting nodal liquid.",0910.1648v1 2009-10-26,Wafer-scale synthesis and transfer of graphene films,"We developed means to produce wafer scale, high-quality graphene films as large as 3 inch wafer size on Ni and Cu films under ambient-pressure and transfer them onto arbitrary substrates through instantaneous etching of metal layers. We also demonstrated the applications of the large-area graphene films for the batch fabrication of field-effect transistor (FET) arrays and stretchable strain gauges showing extraordinary performances. Transistors showed the hole and electron mobilities of the device of 1,100 cm2/Vs and 550 cm2/Vs at drain bias of -0.75V, respectively. The piezo-resistance gauge factor of strain sensor was ~6.1. These methods represent a significant step toward the realization of graphene devices in wafer scale as well as application in optoelectronics, flexible and stretchable electronics.",0910.4783v1 2009-11-25,RETGEM with polyvinylchloride (PVC) electrodes,"This paper presents a new design of the RETGEM (Resistive Electrode Thick GEM) based on electrodes made of a polyvinylchloride material (PVC). Our device can operate with gains of 10E5 as a conventional TGEM at low counting rates and as RPC in the case of high counting rates without of the transit to the violent sparks. The distinct feature of present RETGEM is the absent of the metal coating and lithographic technology for manufacturing of the protective dielectric rms. The electrodes from PVC permit to do the holes by a simple drilling machine. Detectors on a RETGEM basis could be useful in many fields of an application requiring a more cheap manufacturing and safe operation, for example, in a large neutrino experiments, in TPC, RICH systems.",0911.4807v1 2009-12-03,Atomic-scale patterning of hydrogen terminated Ge(001) by scanning tunneling microscopy,"In this paper we demonstrate atomic-scale lithography on hydrogen terminated Ge(001. The lithographic patterns were obtained by selectively desorbing hydrogen atoms from a H resist layer adsorbed on a clean, atomically flat Ge(001) surface with a scanning tunneling microscope tip operating in ultra-high vacuum. The influence of the tip-to-sample bias on the lithographic process have been investigated. Lithographic patterns with feature-sizes from 200 nm to 1.8 nm have been achieved by varying the tip-to-sample bias. These results open up the possibility of a scanning-probe lithography approach to the fabrication of future atomic-scale devices in germanium.",0912.0754v1 2009-12-10,Highly Uniform 300 mm Wafer-Scale Deposition of Single and Multilayered Chemically Derived Graphene Thin Films,"The deposition of atomically thin highly uniform chemically derived graphene (CDG) films on 300 mm SiO2/Si wafers is reported. We demonstrate that the very thin films can be lifted off to form uniform membranes than can be free-standing or transferred onto any substrate. Detailed maps of thickness using Raman spectroscopy and atomic force microscopy (AFM) height profiles reveal that the film thickness is very uniform and highly controllable, ranging from 1-2 layers up to 30 layers. After reduction using a variety of methods, the CDG films are transparent and electrically active with FET devices yielding exceptionally high mobilities of ~ 15 cm2/Vs and sheet resistance of ~ 1 k Ohm/sq at ~ 70 % transparency.",0912.2087v1 2009-12-21,Microstructure and superconductivity of Ir-doped BaFe2As2 superconductor,"Polycrystalline samples with nominal composition of Ba(Fe1-xIrx)2As2 (x=0.10, 0.15, and 0.20) were investigated by means of X-ray diffraction (XRD), scanning electron microscopy (SEM), electrical resistivity, and magnetization measurements. XRD and SEM results showed that almost single phase samples were obtained. Bulk superconductivity with TC~28 K was observed in the x=0.10 sample. TC~28 K is the highest superconducting critical temperature among the reported data for electron-doped AFe2As2-type (A=Ca, Sr, and Ba) superconductors. The upper critical field Hc2(0) reaches as high as 65 T for the x=0.10 sample. The underlying physics is discussed in connection with Co-doping case.",0912.4113v1 2010-01-21,Photon assisted tunneling as an origin of the Dynes density of states,"We show that the effect of a high-temperature environment in current transport through a normal metal-insulator-superconductor tunnel junction can be described by an effective density of states (DOS) in the superconductor. In the limit of a resistive low-ohmic environment, this DOS reduces into the well-known Dynes form. Our theoretical result is supported by experiments in engineered environments. We apply our findings to improve the performance of a single-electron turnstile, a potential candidate for a metrological current source.",1001.3853v3 2010-02-07,Time-Dependent Transport Through Molecular Junctions,"We investigate transport properties of molecular junctions under two types of bias--a short time pulse or an AC bias--by combining a solution for the Green functions in the time domain with electronic structure information coming from ab initio density functional calculations. We find that the short time response depends on lead structure, bias voltage, and barrier heights both at the molecule-lead contacts and within molecules. Under a low frequency AC bias, the electron flow either tracks or leads the bias signal (capacitive or resistive response) depending on whether the junction is perfectly conducting or not. For high frequency, the current lags the bias signal due to the kinetic inductance. The transition frequency is an intrinsic property of the junctions.",1002.1441v1 2010-03-16,All Magnesium diboride Josephson Junctions with MgO and native oxide barriers,"We present results on all-MgB2 tunnel junctions, where the tunnel barrier is deposited MgO or native-oxide of base electrode. For the junctions with MgO, the hysteretic I-V curve resembles a conventional underdamped Josephson junction characteristic with critical current-resistance product nearly independent of the junction area. The dependence of the critical current with temperature up to 20 K agrees with the [Ambegaokar and Baratoff, Phys. Rev. Lett. 10, 486 (1963)] expression. For the junctions with native-oxide, conductance at low bias exhibits subgap features while at high bias reveals thick barriers. As a result no supercurrent was observed in the latter, despite the presence of superconducting-gaps to over 30 K.",1003.3158v1 2010-03-31,Magneto-transport Effects in Topological Insulator Bi$_2$Se$_3$ Nanoribbons,"Magneto-resistance (MR) of Bi$_2$Se$_3$ nanoribbons is studied over a broad range of temperature ($T$=300K-2K) and under various magnetic field ($B$) orientations. The MR is strongly anisotropic with the perpendicular MR much larger than the longitudinal and transverse MRs. The perpendicular MR exhibits quadratic $B$-dependence in low fields and becomes linear at high $B$. However, when $T$ increases, the perpendicular MR becomes linear over the whole magnetic field range (0-9T) up to room temperature. This unusual linear MR is discussed in the context of the linear quantum MR of the topological surface-states. We also observe the boundary-scattering effect in MR at low temperatures, which indicates that the out-of-plane Fermi momentum is much smaller the in-plane Fermi momentum, excluding the simple three-dimensional Fermi surface picture.",1003.6099v4 2010-04-05,Hysteresis in the magneto-transport of Manganese-doped Germanium: evidence for carrier-mediated ferromagnetism,"We report the fabrication of Ge:Mn ferromagnetic semiconductors by Mn-ion implantation into Ge followed by pulsed laser annealing. Benefiting from the short time annealing, the hole concentration in Mn-implanted Ge has been increased by two orders of magnitude from 10$^{18}$ to over 10$^{20}$ cm$^{-3}$. Likely due to the high hole concentration, we observe that the longitudinal and Hall resistances exhibit the same hysteresis as the magnetization, which is usually considered as a sign of carrier-mediated ferromagnetism.",1004.0568v1 2010-04-21,"Effect of pressure on the magnetic, transport, and thermal-transport properties of the electron-doped manganite CaMn$_{1-x}$Sb$_{x}$O$_{3}$","We have demonstrated the effect of hydrostatic pressure on magnetic and transport properties, and thermal transport properties in electron-doped manganites CaMn$_{1-x}$Sb$_{x}$O$_{3}$. The substitution of Sb$^{5+}$ ion for Mn $^{4+}$site of the parent matrix causes one-electron doping with the chemical formula CaMn$^{4+}_{1-2x}$Mn$^{3+}_{x}$Sb$^{5+}_{x}$O$_{3}$ accompanied by a monotonous increase in unit cell volume as a function of $x$. Upon increasing the doping level of Sb, the magnitudes of both electrical resistivity and negative Seebeck coefficient are suppressed at high temperatures, indicating the electron doping. Anomalous diamagnetic behaviors at $x=0.05$ and 0.08 are clearly observed in field cooled dc magnetization. The effect of hydrostatic pressure on dc magnetization is in contrast to the chemical pressure effect due to Sb doping. The dynamical effect of ac magnetic susceptibility measurement points to the formation of the magnetically frustrated clusters such as FM clusters embedded in canted AFM matrix.",1004.3669v3 2010-05-06,Theoretical and Experimental Studies of Schottky Diodes That Use Aligned Arrays of Single Walled Carbon Nanotubes,"We present theoretical and experimental studies of Schottky diodes that use aligned arrays of single walled carbon nanotubes. A simple physical model, taking into account the basic physics of current rectification, can adequately describe the single-tube and array devices. We show that for as grown array diodes, the rectification ratio, defined by the maximum-to-minimum-current-ratio, is low due to the presence of m-SWNT shunts. These tubes can be eliminated in a single voltage sweep resulting in a high rectification array device. Further analysis also shows that the channel resistance, and not the intrinsic nanotube diode properties, limits the rectification in devices with channel length up to ten micrometer.",1005.0870v1 2010-06-16,Perfect Domain-Lattice Matching Between MgB2 and Al2O3: Single-Crystal MgB2 Thin Films Grown on Sapphire,"We have found that single-crystal films can be grown on (0001) Al2O3 substrates through the golden relation of a perfect lattice-matching ratio between the a-axis lattice constants of MgB2 and Al2O3. Selected area electron diffraction patterns evidently indicate hexagonal MgB2 film with a 30 degrees in-plane rotation with respect to the Al2O3 substrate. The films grown on Al2O3 show a zero-resistance transition temperature of 39.6 K with a transition width of 0.1 K. The critical current density at zero field is comparable to the depairing critical current density and rapidly decreases with increasing applied field due to the lack of pinning sites, as observed for high-quality MgB2 single crystals.",1006.3169v1 2010-07-01,Chip-scale nanofabrication of single spins and spin arrays in diamond,"We demonstrate a technique to nanofabricate nitrogen vacancy (NV) centers in diamond based on broad-beam nitrogen implantation through apertures in electron beam lithography resist. This method enables high-throughput nanofabrication of single NV centers on sub-100 nm length scales. Secondary ion mass spectroscopy (SIMS) measurements facilitate depth profiling of the implanted nitrogen to provide three-dimensional characterization of the NV center spatial distribution. Measurements of NV center coherence with on-chip coplanar waveguides suggest a pathway for incorporating this scalable nanofabrication technique in future quantum applications.",1007.0240v2 2010-08-04,Transport in gapped bilayer graphene: the role of potential fluctuations,"We employ a dual-gated geometry to control the band gap \Delta in bilayer graphene and study the temperature dependence of the resistance at the charge neutrality point, RNP(T), from 220 to 1.5 K. Above 5 K, RNP(T) is dominated by two thermally activated processes in different temperature regimes and exhibits exp(T3/T)^{1/3} below 5 K. We develop a simple model to account for the experimental observations, which highlights the crucial role of localized states produced by potential fluctuations. The high temperature conduction is attributed to thermal activation to the mobility edge. The activation energy approaches \Delta /2 at large band gap. At intermediate and low temperatures, the dominant conduction mechanisms are nearest neighbor hopping and variable-range hopping through localized states. Our systematic study provides a coherent understanding of transport in gapped bilayer graphene.",1008.0783v1 2010-09-13,Cooper Pair Writing at the LaAlO3/SrTiO3 Interface,"The LaAlO3/SrTiO3 interface provides a unique platform for controlling the electronic properties of the superconducting semiconductor SrTiO3. Prior investigations have shown that two-dimensional superconductivity can be produced at the LaAlO3/SrTiO3 interface and tuned electrostatically. The recently demonstrated reversible control of the metal-insulator transition at the same interface using conductive atomic force microscopy (c-AFM) raises the question of whether this room-temperature technique can produce structures that exhibit superconducting, normal metallic and insulating phases at sub-Kelvin temperatures. Here we report low-temperature magnetotransport experiments on conducting structures defined at an otherwise insulating LaAlO3/SrTiO3 interface. A quantum phase transition associated with the formation of Cooper pairs is observed in these predefined structures at sub-Kelvin temperatures. However, a finite resistance remains even at the lowest temperature. At higher magnetic fields, interfaces with high mobility also exhibit strong Shubnikov-de Haas oscillations as well as a larger Ginsburg-Landau coherence length. Cooper pair localization, spin-orbit coupling, and finite-size effects may factor into an explanation for some of the unusual properties observed.",1009.2424v2 2010-09-16,Overlapping-gate architecture for silicon Hall bar MOSFET devices in the low electron density regime,"We report the fabrication and study of Hall bar MOSFET devices in which an overlapping-gate architecture allows four-terminal measurements of low-density 2D electron systems, while maintaining a high density at the ohmic contacts. Comparison with devices made using a standard single gate show that measurements can be performed at much lower densities and higher channel resistances, despite a reduced peak mobility. We also observe a voltage threshold shift which we attribute to negative oxide charge, injected during electron-beam lithography processing.",1009.3109v1 2010-10-01,Contactless measurement of electrical conductance of a thin film of amorphous germanium,"We present a contactless method for measuring charge in a thin film of amorphous germanium (a-Ge) with a nanoscale silicon MOSFET charge sensor. This method enables the measurement of conductance of the a-Ge film even in the presence of blocking contacts. At high bias voltage, the resistance of the contacts becomes negligible and a direct measurement of current gives a conductance that agrees with that from the measurement of charge. This charge-sensing technique is used to measure the temperature- and field-dependence of the conductance, and they both agree with a model of Mott variable-range hopping. From the model, we obtain a density of states at the Fermi energy of 1.6 x 10^18 eV^-1 cm^-3 and a localization length of 1.06 nm. This technique enables the measurement of conductance as low as 10^-19 S.",1010.0045v1 2010-10-05,Optical property modification of ZnO: Effect of 1.2 MeV Ar irradiation,"We report a systematic study on 1.2 MeV Ar^8+ irradiated ZnO by x-ray diffraction (XRD), room temperature photoluminescence (PL) and ultraviolet-visible (UV-Vis) absorption measurements. ZnO retains its wurtzite crystal structure up to maximum fluence of 5 x 10^16 ions/cm^2. Even, the width of the XRD peaks changes little with irradiation. The UV-Vis absorption spectra of the samples, unirradiated and irradiated with lowest fluence (1 x 10^15 ions/cm^2), are nearly same. However, the PL emission is largely quenched for this irradiated sample. Red shift of the absorption edge has been noticed for higher fluence. It has been found that red shift is due to at least two defect centers. The PL emission is recovered for 5 x 10^15 ions/cm^2 fluence. The sample colour is changed to orange and then to dark brown with increasing irradiation fluence. Huge resistivity decrease is observed for the sample irradiated with 5 x 10^15 ions/cm^2 fluence. Results altogether indicate the evolution of stable oxygen vacancies and zinc interstitials as dominant defects for high fluence irradiation.",1010.0753v1 2010-11-23,Transport in Graphene Tunnel Junctions,"We present a technique to fabricate tunnel junctions between graphene and Al and Cu, with a Si back gate, as well as a simple theory of tunneling between a metal and graphene. We map the differential conductance of our junctions versus probe and back gate voltage, and observe fluctuations in the conductance that are directly related to the graphene density of states. The conventional strong-suppression of the conductance at the graphene Dirac point can not be clearly demonstrated, but a more robust signature of the Dirac point is found: the inflection in the conductance map caused by the electrostatic gating of graphene by the tunnel probe. We present numerical simulations of our conductance maps, confirming the measurement results. In addition, Al causes strong n-doping of graphene, Cu causes a moderate p-doping, and in high resistance junctions, phonon resonances are observed, as in STM studies.",1011.5067v1 2010-12-14,Reentrant spin-glass behavior in $TlFe_{2-x}Se_2$ with the $ThCr_2Si_2$-type structure,"We investigated the physical properties of $TlFe_{2-x}Se_2$ single crystals. The resistivity of $TlFe_{2-x}Se_2$ shows typical semiconductor behavior with an activation energy of 25 meV. DC susceptibility indicates an antiferromagnetic transition at about 450 K. Reentrant spin-glass (RSG) behavior was found at about 130 K through DC and AC magnetic measurements. The RSG behavior suggests the existence of a strong competition between ferromagnetic (FM) and antiferromagnetic (AFM) interactions due to Fe deficiencies. Strong electron-electron correlation may exist in this material and it is possibly a candidate of parent compound for high $T_c$ superconductors.",1012.2929v1 2010-12-23,Effect of chromium disorder on the thermoelectric properties of Layered-antiferromagnet CuCrS2,"Layered-antiferromagnetic compound CuCrS2 has been prepared by different methods. The analysis of X-ray diffraction patterns of different samples gave significant amount of vacancy-disorder of Cr-atoms within the layers. Extended period of sintering above 9000C increases the transfer of Cr-atoms to the interstitial sites between the layers. This disorder has marginal effect on the Antiferromagnetic properties. The electrical conductivity is increased and the thermoelectric power remains positive and quite high between 150-400\muV/K in the paramagnetic state around room temperature with increase in disorder in different samples. We interpret the temperature dependence of electrical resistivity and thermoelectric power due to the localization of carriers by interstitial defects and the formation of magnetic polarons in the paramagnetic phase of CuCrS2.",1012.5147v1 2011-03-04,Giant enhancement of spin accumulation and long-distance spin precession in metallic lateral spin valves,"The nonlocal spin injection in lateral spin valves is highly expected to be an effective method to generate a pure spin current for potential spintronic application. However, the spin valve voltage, which decides the magnitude of the spin current flowing into an additional ferromagnetic wire, is typically of the order of 1 {\mu}V. Here we show that lateral spin valves with low resistive NiFe/MgO/Ag junctions enable the efficient spin injection with high applied current density, which leads to the spin valve voltage increased hundredfold. Hanle effect measurements demonstrate a long-distance collective 2-pi spin precession along a 6 {\mu}m long Ag wire. These results suggest a route to faster and manipulable spin transport for the development of pure spin current based memory, logic and sensing devices.",1103.0852v2 2011-03-23,Local Electrical Stress-Induced Doping and Formation of 2D Monolayer Graphene P-N Junction,"We demonstrated doping in 2D monolayer graphene via local electrical stressing. The doping, confirmed by the resistance-voltage transfer characteristics of the graphene system, is observed to continuously tunable from N-type to P-type as the electrical stressing level (voltage) increases. Two major physical mechanisms are proposed to interpret the observed phenomena: modifications of surface chemistry for N-type doping (at low-level stressing) and thermally-activated charge transfer from graphene to SiO2 substrate for P-type doping (at high-level stressing). The formation of P-N junction on 2D graphene monolayer is demonstrated with complementary doping based on locally applied electrical stressing.",1103.4568v3 2011-03-25,Giant Positive Magnetoresistance in Co@CoO Nanoparticle Arrays,"We report the magnetotransport properties of self-assembled Co@CoO nanoparticle arrays at temperatures below 100 K. Resistance shows thermally activated behavior that can be fitted by the general expression of R exp{(T/T0)^v}. Efros-Shklovskii variable range hopping (v=1/2) and simple activation (hard gap, v=1) dominate the high and low temperature region, respectively, with a strongly temperature-dependent transition regime in between. A giant positive magnetoresistance of >1,400% is observed at 10K, which decreases with increasing temperature. The positive MR and most of its features can be explained by the Zeeman splitting of the localized states that suppresses the spin dependent hopping paths in the presence of on-site Coulomb repulsion.",1103.5029v1 2011-05-06,Optical excitation of Electron-Glasses,"Electron-glasses can be readily driven far from equilibrium by a variety of means. Several mechanisms to excite the system and their relative merits are reviewed. In this study we focus on the process of exciting electron-glasses by interaction with near infrared radiation. The efficiency of this protocol varies considerably among different electron-glasses, but it only weakly depends on their resistance at liquid helium temperatures. A dramatic enhancement of the excitation efficiency is observed upon doping crystalline indium-oxide with Au. Some enhancement is observed also in samples doped with Pb but this enhancement fades away with time unlike the situation in the Au-doped samples. Several structural and analytical tools are used to characterize the changes in the materials that may be responsible for these effects. Possible routes by which high-frequency electromagnetic fields take the system far from equilibrium are discussed.",1105.1350v1 2011-05-22,Evidence for a capacitor network near the metal insulator transition in VO2 thin films probed by in-plane impedance spectroscopy,"Impedance spectroscopy measurements were performed in high quality Vanadium dioxide (VO2) thin films. This technique allows us investigate the resistive and capacitive contribution to the dielectric response near the metal-insulator transition (MIT). A non ideal RC behavior was found in our films from room temperature up to 334 K. A decrease of the total capacitance was found in this region, possibly due to interface effects. Above the MIT, the system behaves like a metal as expected, and a modified equivalent circuit is necessary to describe the impedance data adequately. Around the MIT, an increase of the total capacitance is observed.",1105.4308v1 2011-05-24,Rectification at Graphene-Semiconductor Interfaces: Zero-Gap Semiconductor Based Diodes,"Using current-voltage (I-V) and capacitance-voltage (C-V) measurements, we report on the unusual physics and promising technical applications associated with the formation of Schottky barriers at the interface of a one-atom-thick zero-gap semiconductor (graphene) and conventional semiconductors. When chemical vapor deposited graphene is transferred onto n-type Si, GaAs, 4H-SiC and GaN semiconductor substrates, there is a strong van der Waals attraction that is accompanied by charge transfer across the interface and the formation of a rectifying (Schottky) barrier. Thermionic emission theory in conjunction with the Schottky-Mott model within the context of bond-polarization theory provides a surprisingly good description of the electrical properties. Applications, such as to sensors where in forward bias there is exponential sensitivity to changes in the Schottky barrier height due to the presence of absorbates on the graphene or to analogue devices for which Schottky barriers are integral components are promising because of graphene's mechanical stability, its resistance to diffusion, its robustness at high temperatures and its demonstrated capability to embrace multiple functionalities.",1105.4811v2 2011-05-27,"Magnonic spin-transfer torque MRAM with low power, high speed, and error-free switching","A new class of spin-transfer torque magnetic random access memory (STT-MRAM) is discussed, in which writing is achieved using thermally initiated magnonic current pulses as an alternative to conventional electric current pulses. The magnonic pulses are used to destabilize the magnetic free layer from its initial direction, and are followed immediately by a bipolar electric current exerting conventional spin-transfer torque on the free layer. The combination of thermal and electric currents greatly reduces switching errors, and simultaneously reduces the electric switching current density by more than an order of magnitude as compared to conventional STT-MRAM. The energy efficiency of several possible electro-thermal circuit designs have been analyzed numerically. As compared to STT-MRAM with perpendicular magnetic anisotropy, magnonic STT-MRAM reduces the overall switching energy by almost 80%. Furthermore, the lower electric current density allows the use of thicker tunnel barriers, which should result in higher tunneling magneto-resistance and improved tunnel barrier reliability. The combination of lower power, improved reliability, higher integration density, and larger read margin make magnonic STT-MRAM a promising choice for future non-volatile storage.",1105.5473v1 2011-05-27,Temperature Dependence of the Intrinsic Anomalous Hall Effect in Nickel,"We investigate the unusual temperature dependence of the anomalous Hall effect in Ni. By varying the thickness of the MBE-grown Ni films, the longitudinal resistivity is uniquely tuned without resorting to doping impurities; consequently, the intrinsic and extrinsic contributions are cleanly separated out. In stark contrast to other ferromagnets such as Fe, the intrinsic contribution in Ni is found to be strongly temperature dependent with a value of 1100 (ohm*cm)^(-1) at low temperatures and 500 (ohm*cm)^(-1) at high temperatures. This pronounced temperature dependence, a cause of long-standing confusion concerning the physical origin of the AHE, is likely due to the small energy level splitting caused by the spin orbit coupling close to the Fermi surface. Our result helps pave the way for the general claim of the Berry-phase interpretation for the AHE.",1105.5664v1 2011-05-31,Interplay between topological insulators and superconductors,"Topological insulators are insulating in the bulk but possess metallic surface states protected by time-reversal symmetry. Here, we report a detailed electronic transport study in high quality Bi2Se3 topological insulator thin films contacted by superconducting (In, Al and W) electrodes. The resistance of the film shows an abrupt and significant upturn when the electrodes become superconducting. In turn, the Bi2Se3 film strongly weakens the superconductivity of the electrodes, significantly reducing both their transition temperatures and critical fields. A possible interpretation of these results is that the superconducting electrodes are accessing the surface states and the experimental results are the consequence of the interplay between the Cooper pairs of the electrodes and the spin polarized current of the surface states in Bi2Se3.",1105.6174v3 2011-06-04,Facile fabrication of lateral nanowire wrap-gate devices with improved performance,"We present a simple fabrication technique for lateral nanowire wrap-gate devices with high capacitive coupling and field-effect mobility. Our process uses e-beam lithography with a single resist-spinning step, and does not require chemical etching. We measure, in the temperature range 1.5-250 K, a subthreshold slope of 5-54 mV/decade and mobility of 2800-2500 $cm^2/Vs$ -- significantly larger than previously reported lateral wrap-gate devices. At depletion, the barrier height due to the gated region is proportional to applied wrap-gate voltage.",1106.0796v1 2011-06-04,Mechanochemical reaction in graphane under uniaxial tension,"The quantum-mechanochemical-reaction-coordinate simulations have been performed to investigate the mechanical properties of hydrogen functionalized graphene. The simulations disclosed atomically matched peculiarities that accompany the deformation-failure-rupture process occurred in the body. A comparative study of the deformation peculiarities related to equi-carbon-core (5,5) nanographene and nanographane sheets exhibited a high stiffness of both bodies that is provided by the related hexagon units, namely benzenoid and cyclohexanoid, respectively. The two units are characterized by anisotropy in the microscopic behavior under elongation along mechanochemical internal coordinates when the later are oriented either along (zg) or normally (ach) to the C-C bonds chain. The unit feature in combination with different configuration of their packing with respect to the body C-C bond chains forms the ground for the structure-sensitive mechanical behavior that is different for zg and ach deformation modes. Hydrogenation of graphene drastically influences behavior and numerical characteristics of the body making tricotage-like pattern of the graphene failure less pronounced and inverting it from the zg to ach mode as well as providing less mechanical resistance of graphane it total.",1106.0837v2 2011-07-09,Huge Volume Expansion and Structural Transformation of Carbon Nanotube Aligned Arrays during Electrical Breakdown in Vacuum,"We observed a huge volume expansion of aligned single walled carbon nanotube (SWNT) arrays accompanied by structural transformation during electrical breakdown in vacuum. The SWNT arrays were assembled between prefabricated Pd source and drain electrodes of 2 \mu m separation on Si/SiO_2 substrate via dielectrophoresis. At high electrical field, the SWNT arrays erupt into large mushroom-like structure. Systematic studies with controlled electrical bias show that above a certain field SWNTs swell and transform to nanoparticles and flower-like structures with small volume increase. Further increase in electrical bias and repeated sweeping results into amorphous carbon as determined from scanning and transmission electron microscopy (TEM). Cross sectional studies using focused ion beam and TEM show the height of 2-3 nm SWNT array increased to about 1 \mu m with a volume gain of ~ 400 times. The electron energy loss spectroscopy reveals that graphitic sp^2 networks of SWNTs are transformed predominantly to sp^3. The current-voltage measurements also show an increase in the resistance of the transformed structure.",1107.1758v1 2011-07-20,Macroscopic Superconducting Current through a Silicon Surface Reconstruction with Indium Adatoms: Si(111)-(R7$\times$R3)-In,"Macroscopic and robust supercurrents are observed by direct electron transport measurements on a silicon surface reconstruction with In adatoms (Si(111)-(R7xR3)-In). The superconducting transition manifests itself as an emergence of the zero resistance state below 2.8 K. $I-V$ characteristics exhibit sharp and hysteretic switching between superconducting and normal states with well-defined critical and retrapping currents. The two-dimensional (2D) critical current density $J_\mathrm{2D,c}$ is estimated to be as high as $1.8 \ \mathrm{A/m}$ at 1.8 K. The temperature dependence of $J_\mathrm{2D,c}$ indicates that the surface atomic steps play the role of strongly coupled Josephson junctions.",1107.3902v2 2011-07-30,Indications of an Electronic Phase Transition in 2D YBa2Cu3O7-x Induced by Electrostatic Doping,"We successfully tuned an underdoped ultrathin YBa2Cu3O7-x film into the overdoped regime by means of electrostatic doping using an ionic liquid as a dielectric material. This process proved to be reversible. Transport measurements showed a series of anomalous features compared to chemically doped bulk samples and a different two-step doping mechanism for electrostatic doping was revealed. The normal resistance increased with carrier concentration on the overdoped side and the high temperature (180 K) Hall number peaked at a doping level of p$\sim$0.15. These anomalous behaviors suggest that there is an electronic phase transition in the Fermi surface around the optimal doping level.",1108.0083v1 2011-08-01,Evolution of Structural and Physical Properties of Sr3(Ru1-xMnx)2O7 with Mn Concentration,"Layered ruthenates are prototype materials with strong structure-property correlations. We report the structural and physical properties of double-layered perovskite Sr3(Ru1-xMnx)2O7 single crystals with 0<=x<=0.7. Single crystal x-ray diffraction refinements reveal that Mn doping on the Ru site leads to the shrinkage of unit-cell volume and disappearance of (Ru/Mn)O6 octahedron rotation when x>0.16, while the crystal structure remains tetragonal. Correspondingly, the electric and magnetic properties change with x. The electrical resistivity reveals metallic character (d rho/d T>0) at high temperatures but insulating behavior (d rho/d T<0) below a characteristic temperature T_MIT. Interestingly, T_MIT is different from T_M, at which magnetic susceptibility reaches maximum. T_MIT monotonically increases with increasing x while T_M shows non-monotonic dependence with x. The difference between T_MIT and T_M (T_MIT>T_M) becomes larger when x>0.16. The constructed phase diagram consists of five distinct regions, demonstrating that the physical properties of such a system can easily be tuned by chemical doping.",1108.0392v1 2011-08-15,Large conductance modulation of gold thin films by huge charge injection via electrochemical gating,"By using an electrochemical gating technique with a new combination of polymer and electrolyte, we were able to inject surface charge densities n_2D as high as 3.5 \times 10^15 e/cm^2 in gold films and to observe large relative variations in the film resistance, DeltaR/R', up to 10% at low temperature. DeltaR/R' is a linear function of n_2D - as expected within a free-electron model - if the film is thick enough (> 25 nm), otherwise a tendency to saturation due to size effects is observed. The application of this technique to 2D materials will allow extending the field-effect experiments to a range of charge doping where giant conductance modulations and, in some cases, even the occurrence of superconductivity are expected.",1108.3099v1 2011-09-19,Fe-doping induced superconductivity in charge-density-wave system 1T-TaS2,"We report the interplay between charge-density-wave (CDW) and superconductivity of 1$T$-Fe$_{x}$Ta$_{1-x}$S$_{2}$ ($0\leq x \leq 0.05$) single crystals. The CDW order is gradually suppressed by Fe-doping, accompanied by the disappearance of pseudogap/Mott-gap as shown by the density functional theory (DFT) calculations. The superconducting state develops at low temperatures within the CDW state for the samples with the moderate doping levels. The superconductivity strongly depends on $x$ within a narrow range, and the maximum superconducting transition temperature is 2.8 K as $x=0.02$. We propose that the induced superconductivity and CDW phases are separated in real space. For high doping level ($x>0.04$), the Anderson localization (AL) state appears, resulting in a large increase of resistivity. We present a complete electronic phase diagram of 1$T$-Fe$_{x}$Ta$_{1-x}$S$_{2}$ system that shows a dome-like $T_{c}(x)$.",1109.3962v3 2011-09-28,A combination of capillary assembly and dielectrophoresis for wafer scale integration of carbon nanotubes-based electrical and mechanical devices,"The wafer scale integration of carbon nanotubes (CNT) remains a challenge for electronic and electromechanical applications. We propose a novel CNT integration process relying on the combination of controlled capillary assembly and buried electrode dielectrophoresis (DEP). This process enables to monitor the precise spatial localization of a high density of CNTs and their alignment in a pre-defined direction. Large arrays of independent and low resistivity (4.4 x 10^-5 {\Omega}.m) interconnections were achieved using this hybrid assembly with double-walled carbon nanotubes (DWNT). Finally, arrays of suspended individual CNT carpets have been realized and we demonstrate their potential use as functional nano-electromechanical systems (NEMS) by monitoring their resonance frequencies (ranging between 1.7 MHz to 10.5MHz) using a Fabry-Perot interferometer.",1109.6268v1 2011-11-14,Thermoelectric properties of Ba-Cu-Si clathrates,"Thermoelectric properties of the type-I clathrates Ba$_8$Cu$_x$Si$_{46-x}$ ($3.6 \leq x \leq 7$, $x$ = nominal Cu content) are investigated both experimentally and theoretically. The polycrystalline samples are prepared either by melting, ball milling and hot pressing or by melt spinning, hand milling and hot pressing techniques. Temperature-dependent electrical resistivity, $\rho(T)$, and the Seebeck coefficient, $S(T)$, measurements reveal metal-like behavior for all samples. For $x = 5$ and 6, density functional theory calculations are performed for deriving the enthalpy of formation and the electronic structure which is exploited for the calculation of Seebeck coefficients and conductivity within Boltzmann's transport theory. For simulating the properties of doped clathrates the rigid band model is applied. On the basis of the density functional theory results the experimentally observed compositional dependence of $\rho(T)$ and $S(T)$ of the whole sample series is analyzed. The highest dimensionless thermoelectric figure of merit $ZT$ of 0.28 is reached for a melt-spun sample at $600^{\circ}$C. The relatively low $ZT$ values in this system are attributed to the too high charge carrier concentrations.",1111.3278v1 2011-12-13,The Disordered Induced Interaction and the Phase Diagram of Cuprates,"There are processes in nature that resemble a true force but arise due to the minimization of the local energy. The most well-known case is the exchange interaction that leads to magnetic order in some materials. We discovered a new similar process occurring in connection with an electronic phase separation transition that leads to charge inhomogeneity in cuprate superconductors. The minimization of the local free energy, described here by the Cahn-Hilliard diffusion equation, drives the charges into regions of low and high densities. This motion leads to an effective potential with two-fold effect: creation of tiny isolated regions or micrograins, and two-body attraction, which promotes local or intra-grain superconducting pairing. Consequently, as in granular superconductors, the superconducting transition appears in two steps. First, with local intra-grain superconducting amplitudes and, at lower temperature, the superconducting phase or resistivity transition is attained by intergrain Josephson coupling. We show here that this approach reproduces the main features of the cuprates phase diagram, gives a clear interpretation to the pseudogap phase and yields the position dependent local density of states gap $\Delta(\vec r)$ measured by tunnelling experiments.",1112.2880v1 2012-05-08,Normal and intrinsic anomalous Hall effect in Nb1-yFe2+y,"The Hall effect on selected samples of the dilution series Nb1-yFe2+y is studied. Normal and anomalous contributions are observed, with positive normal Hall effect dominating at high temperatures. Consistent analysis of the anomalous contribution is only possible for Fe-rich Nb0.985Fe2.015 featuring a ferromagnetic ground state. Here, a positive normal Hall coefficient is found at all temperatures with a moderate maximum at the spin-density-wave transition. The anomalous Hall effect is consistent with an intrinsic (Berry-phase) contribution which is constant below the ordering temperature TC and continuously vanishes above TC. For stoichiometric NbFe2 and Nb-rich Nb1.01Fe1.99 - both having a spin-density-wave ground state - an additional contribution to the Hall resistivity impedes a complete analysis and indicates the need for more sophisticated models of the anomalous Hall effect in itinerant antiferromagnets.",1205.1651v1 2012-05-10,Physical properties and crystal chemistry of Ce2Ga12Pt,"Single crystals of the new ternary compound Ce2Ga12Pt were prepared by the self-flux technique. The crystal structure with the space group P4/nbm was established from single-crystal X-ray diffraction data and presents a derivative of the LaGa6Ni0.6 prototype. Magnetic susceptibility measurements show Curie-Weiss behaviour due to local Ce^3+ moments. At high temperatures, the magnetic anisotropy is dominated by the crystal-electric-field (CEF) effect with the easy axis along the crystallographic c direction. Ce2Ga12Pt undergoes two antiferromagnetic phase transitions at T_N,1 = 7.3K and T_N,2 = 5.5K and presents several metamagnetic transitions for the magnetic field along c. Specific-heat measurements prove the bulk nature of these magnetic transitions and reveal a doublet CEF ground state. The 4f contribution to the resistivity shows a broad maximum at T_max ~ 85K due to Kondo scattering off the CEF ground state and excited levels.",1205.2301v1 2012-05-13,Voltage-Induced Ferromagnetic Resonance in Magnetic Tunnel Junctions,"We demonstrate excitation of ferromagnetic resonance in CoFeB/MgO/CoFeB magnetic tunnel junctions (MTJs) by the combined action of voltage-controlled magnetic anisotropy (VCMA) and spin transfer torque (ST). Our measurements reveal that GHz-frequency VCMA torque and ST in low-resistance MTJs have similar magnitudes, and thus that both torques are equally important for understanding high-frequency voltage-driven magnetization dynamics in MTJs. As an example, we show that VCMA can increase the sensitivity of an MTJ-based microwave signal detector to the sensitivity level of semiconductor Schottky diodes.",1205.2835v2 2012-05-15,Field-induced high coercive ferromagnetic state and magnetoresistance in the antiferromagnetically ordered compound Fe0.5TiS2,"The measurements of the magnetic susceptibility, magnetization, electrical resistivity and magnetoresistance have been performed for the Fe intercalated compound Fe0.5TiS2. According to X-ray diffraction measurements the Fe0.5TiS2 compound synthesized in the present work has a monoclinic crystal structure (space group I12/m1) which results from the ordering of Fe ions and vacancies between S-Ti-S tri-layres. The changes in the heat-treatment conditions at temperatures below 1100 Celsius degrees do not lead to an order-disorder transition within the subsystem of intercalated Fe ions. It has been shown that this compound exhibits an antiferromagnetic (AF) ground state below the Neel temperature TN = 140 K. Application of the magnetic field at T < TN induces a metamagnetic phase transition to the ferromagnetic (F) state, which is accompanied by the large magnetoresistance effect (up to 27 %). The field-induced AF-F transition is found to be irreversible below ~ 100 K. The magnetization reversal in the metastable F state at low temperatures is accompanied by substantial hysteresis (~ 100 kOe) which is associated with the Ising character of Fe ions.",1205.3242v1 2012-05-16,A new approach for improving global critical current density in Fe(Se0.5Te0.5) polycrystalline materials,"A novel method to prepare bulk Fe(Se0.5Te0.5) samples is presented, based on a melting process and a subsequent annealing treatment. With respect to the standard sintering technique, it produces much more homogeneous and denser samples, characterized by large and well interconnected grains. The resulting samples exhibit optimal critical temperature values, sharp resistive and magnetic transitions, large magnetic hysteresis loops and high upper critical fields are observed. Interestingly, the global critical current density is much enhanced as compared to the values reported in literature for bulk samples of the same 11 family, reaching about 103 A/cm2 at zero field at 4.2 K as assessed by magnetic, transport and magneto-optical techniques. Even more importantly, its field dependence turns out to be very weak, such that at \mu_{0}H = 7 T it is suppressed only by a factor \sim2.",1205.3618v2 2012-05-29,Transformation Electronics: Tailoring Electron's Effective Mass,"The speed of integrated circuits is ultimately limited by the mobility of electrons or holes, which depend on the effective mass in a semiconductor. Here, building on an analogy with electromagnetic metamaterials and transformation optics, we describe a new transport regime in a semiconductor superlattice characterized by extreme anisotropy of the effective mass and a low intrinsic resistance to movement - with zero effective mass - along some preferred direction of electron motion. We theoretically demonstrate that such regime may permit an ultra fast, extremely strong electron response, and significantly high conductivity, which, notably may be weakly dependent on the temperature at low temperatures. These ideas may pave the way for faster electronic devices and detectors and new functional materials with a strong electrical response in the infrared regime.",1205.6325v2 2012-07-13,Association of indigo with zeolites for improved colour stabilization,"The durability of an organic colour and its resistance against external chemical agents and exposure to light can be significantly enhanced by hybridizing the natural dye with a mineral. In search for stable natural pigments, the present work focuses on the association of indigo blue with several zeolitic matrices (LTA zeolite, mordenite, MFI zeolite). The manufacturing of the hybrid pigment is tested under varying oxidising conditions, using Raman and UV-visible spectrometric techniques. Blending indigo with MFI is shown to yield the most stable composite in all of our artificial indigo pigments. In absence of defects and substituted cations such as aluminum in the framework of the MFI zeolite matrix, we show that matching the pore size with the dimensions of the guest indigo molecule is the key factor. The evidence for the high colour stability of indigo@MFI opens a new path for modeling the stability of indigo in various alumino-silicate substrates such as in the historical Maya Blue pigment.",1207.3236v1 2012-08-09,The role of charge traps in inducing hysteresis: capacitance - voltage measurements on top gated bilayer graphene,"Understanding the origin of hysteresis in the channel resistance from top gated graphene transistors is important for transistor applications. Capacitance - voltage measurements across the gate oxide on top gated bilayer graphene show hysteresis with a charging and discharging time constant of ~100 {\mu}s. However, the measured capacitance across the graphene channel does not show any hysteresis, but shows an abrupt jump at a high channel voltage due to the emergence of an order, indicating that the origin of hysteresis between gate and source is due to charge traps present in the gate oxide and graphene interface.",1208.1831v1 2012-08-15,A GEANT4 Simulation Studyof BESIII endcap TOF Upgrade,"A GEANT4-based Monte-Carlo model is developed to study the performance of Endcap Time-Of-Flight (ETOF) at BESIII. It's found that the multiple scattering effects, mainly from the materials at the MDC endcap, can cause multi-hit on the ETOF's readout cell and significantly influence the timing property of ETOF. Multi-gap Resistive Plate Chamber (MRPC) with a smaller readout cell structure is more suitable for ETOF detector due to significantly reduced multi-hit rate, from 71.5% for currently-used scintillator-based ETOF to 21.8% or 16.7% for MRPC-based ETOF, depending on the readout pad size used. The timing performance of a MRPC ETOF is also improved. These simulation results suggest and guide an ETOF upgrade effort at BESIII.",1208.3049v1 2012-09-03,High Efficiency Graphene Solar Cells by Chemical Doping,"We demonstrate single layer graphene/n-Si Schottky junction solar cells that under AM1.5 illumination exhibit a power conversion efficiency (PCE) of 8.6%. This performance, achieved by doping the graphene with bis(trifluoromethanesulfonyl)amide, exceeds the native(undoped) device performance by a factor of 4.5 and the best previously reported PCE in similar devices by a factor of nearly 6. Current-voltage, capacitance-voltage and external quantum efficiency measurements show the enhancement to be due to the doping induced shift in the graphene chemical potential which increases the graphene carrier density (decreasing the cell series resistance) and increases the built-in potential.",1209.0432v1 2012-09-12,Channel Length Scaling of MoS2 MOSFETs,"In this article, we investigate electrical transport properties in ultrathin body (UTB) MoS2 two-dimensional (2D) crystals with channel lengths ranging from 2 {\mu}m down to 50 nm. We compare the short channel behavior of sets of MOSFETs with various channel thickness, and reveal the superior immunity to short channel effects of MoS2 transistors. We observe no obvious short channel effects on the device with 100 nm channel length (Lch) fabricated on a 5 nm thick MoS2 2D crystal even when using 300 nm thick SiO2 as gate dielectric, and has a current on/off ratio up to ~109. We also observe the on-current saturation at short channel devices with continuous scaling due to the carrier velocity saturation. Also, we reveal the performance limit of short channel MoS2 transistors is dominated by the large contact resistance from the Schottky barrier between Ni and MoS2 interface, where a fully transparent contact is needed to achieve a high-performance short channel device.",1209.2525v1 2012-09-24,Ba1-xNaxTi2Sb2O (0.0 <= x <= 0.33): A Layered Titanium-based Pnictide Oxide Superconductor,"A new layered Ti-based pnictide oxide superconductor, Ba1-xNaxTi2Sb2O (0.0 <= x <= 0.33), is reported. X-ray studies reveal it crystallizes in the tetragonal CeCr2Si2C structure. The undoped parent compound, BaTi2Sb2O (P4/mmm; a=4.1196(1){\AA}; c=8.0951(2){\AA}), exhibits a CDW/SDW transition at 54K. Upon chemical doping with Na, the CDW/SDW transition is systematically suppressed and super-conductivity arises with the critical temperatures, Tc, increasing to 5.5 K. Bulk superconductivity is confirmed by resistivity, magnetic and heat capacity measurements. Like the high-Tc cuprates and the iron pnictides, superconductivity in BaTi2Sb2O arises from an ordered state. Similarities and differences to the cuprate and iron pnictide supercon-ductors are discussed.",1209.5447v2 2012-09-27,Fabrication and characterization of semiconducting half Heusler YPtSb thin films,"The semiconducting half Heusler compound YPtSb was predicted theoretically to be capable of changing into topological insulator under proper strain. In this work, p type semiconducting half-Heusler YPtSb thin films were prepared by magnetron co-sputtering method from a specially designed target for the first time. Textured structure with (111) plane paralleling with (001) of MgO substrate was observed when YPtSb thin films were grown on MgO (100) substrate at 600{\deg}C.Electrical measurements show that the resistivity of YPtSb films decreases with increasing temperature, indicating a semiconductor-like behavior. The carrier density is as high as 1.15 X 10^21 cm-3 at 300 K. The band gap of YPtSb thin films obtained by infrared spectroscopy is around 0.1 - 0.15 eV, which is well in agreement with the theoretical prediction and the value measured in bulk YPtSb.",1209.6288v2 2012-10-08,Phonon thermal transport outside of local equilibrium in nanowires via molecular dynamics,"We study thermal transport through Pt nanowires that bridge planar contacts as a function of wire length and vibrational frequency of the contacts. When phonons in the contacts have lower average frequencies than those in the wires thermal transport occurs under conditions away from local equilibrium with low-frequency phonons experiencing a higher thermal gradient than high-frequency ones. This results in a size-dependent increase in the effective thermal conductivity of the wire with decreasing vibrational frequencies of the contacts. The interfacial resistivity when heat flows from the wire to the contact is also size-dependent and has the same physical origin in the lack of full equilibration in short nanowires. We develop a model based on a 1D atomic chain that captures the salient physics of the MD results.",1210.2321v1 2012-10-19,Self-aligned graphene field-effect transistors with polyethyleneimine doped source/drain access regions,"We report a method of fabricating self-aligned, top-gated graphene field-effect transistors (GFETs) employing polyethyleneimine spin-on-doped source/drain access regions, resulting in a 2X reduction of access resistance and a 2.5X improvement in device electrical characteristics, over undoped devices. The GFETs on Si/SiO$_2$ substrates have high carrier mobilities of up to 6,300 cm$^2$/Vs. Self-aligned spin-on-doping is applicable to GFETs on arbitrary substrates, as demonstrated by a 3X enhancement in performance for GFETs on insulating quartz substrates, which are better suited for radio frequency applications.",1210.5535v2 2012-10-22,Fabrication and characterization of the gapless half-Heusler YPtSb thin films,"Half-Heusler YPtSb thin films were fabricated by magnetron co-sputtering method on MgO-buffered SiO2/Si(001) substrates. X-ray diffraction pattern and Energy dispersive X-ray spectroscopy confirmed the high-quality growth and stoichiometry. The temperature dependence of the resistivity shows a semiconducting-type behavior down to low temperature. The Hall mobility was determined to be 450 cm2/Vs at 300K, which is much higher than the bulk value (300 cm2/Vs). In-plane magnetoresistance (MR) measurements with fields applied along and perpendicular to the current direction show opposite MR signs, which suggests the possible existence of the topological surface states.",1210.5808v1 2012-10-29,Impact of graphene quantum capacitance on transport spectroscopy,"We demonstrate experimentally that graphene quantum capacitance $C_{\mathrm{q}}$ can have a strong impact on transport spectroscopy through the interplay with nearby charge reservoirs. The effect is elucidated in a field-effect-gated epitaxial graphene device, in which interface states serve as charge reservoirs. The Fermi-level dependence of $C_{\mathrm{q}}$ is manifested as an unusual parabolic gate voltage ($V_{\mathrm{g}}$) dependence of the carrier density, centered on the Dirac point. Consequently, in high magnetic fields $B$, the spectroscopy of longitudinal resistance ($R_{xx}$) vs. $V_{\mathrm{g}}$ represents the structure of the unequally spaced relativistic graphene Landau levels (LLs). $R_{xx}$ mapping vs. $V_{\mathrm{g}}$ and $B$ thus reveals the vital role of the zero-energy LL on the development of the anomalously wide $\nu=2$ quantum Hall state.",1210.7601v1 2012-11-02,Interface characterization of Co2MnGe/Rh2CuSn Heusler multilayers,"All-Heusler multilayer structures have been investigated by means of high kinetic x-ray photoelectron spectroscopy and x-ray magnetic circular dichroism, aiming to address the amount of disorder and interface diffusion induced by annealing of the multilayer structure. The studied multilayers consist of ferromagnetic Co$_2$MnGe and non-magnetic Rh$_2$CuSn layers with varying thicknesses. We find that diffusion begins already at comparably low temperatures between 200 $^{\circ}$C and 250 $^{\circ}$C, where Mn appears to be most prone to diffusion. We also find evidence for a 4 {\AA} thick magnetically dead layer that, together with the identified interlayer diffusion, are likely reasons for the small magnetoresistance found for current-perpendicular-to-plane giant magneto-resistance devices based on this all-Heusler system.",1211.0489v2 2012-11-13,The giant plasticity of a quantum crystal,"When submitted to large stresses at high temperature, usual crystals may irreversibly deform. This phenomenon is known as plasticity and it is due to the motion of crystal defects such as dislocations. We have discovered that, in the absence of impurities and in the zero temperature limit, helium 4 crystals present a giant plasticity that is anisotropic and reversible. Direct measurements on oriented single crystals show that their resistance to shear nearly vanishes in one particular direction because dislocations glide freely parallel to the basal planes of the hexagonal structure. This plasticity disappears as soon as traces of helium 3 impurities bind to the dislocations or if their motion is damped by collisions with thermal phonons.",1211.2976v2 2012-11-14,High-temperature structural phase transition in multiferroic LiCu_2O_2,"LiCu_2O_2 single crystals were studied in the temperature range 300-1100 K by means of heating-cooling curves of differential thermal analysis (DTA), thermogravimetry (TG), X-ray powder diffraction and electrical measurements. A reversible first-order phase transition between orthorhombic and tetragonal phases was found to take place at 993 K. At the transition, a peak is observed in the DTA curves, as well as jumps of the unit cell parameters and electrical resistivity. Considering the crystal structure of LiCu_2O_2 and the entropy change associated with the phase transition, it is concluded that the phase transition is related to processes of order-disorder of the Cu2+ and Li+ cations onto their crystallographic positions.",1211.3275v1 2012-11-14,Anisotropy and directional pinning in YBaCuO with BaZrO3 nanorods,"Measurements of anisotropic transport properties (dc and high-frequency regime) of driven vortex matter in YBa$_2$Cu$_3$O$_{7-x}$ with elongated strong-pinning sites (c-axis aligned, self-assembled BaZrO$_3$ nanorods) are used to demonstrate that the effective-mass angular scaling takes place only in intrinsic physical quantities (flux-flow resistivity), and not in pinning-related Labusch parameter and critical currents. Comparison of the dynamics at different time scales shows evidence for a transition of the vortex matter toward a Mott phase, driven by the presence of nanorods. The strong pinning in dc arises partially from a dynamic effect.",1211.3311v2 2012-11-23,1D to 3D Dimensional Crossover in the Superconducting Transition of the Quasi-One-Dimensional Carbide Superconductor Sc3CoC4,"The transition metal carbide superconductor Sc3CoC4 may represent a new benchmark system of quasi-1D superconducting behavior. We investigate the superconducting transition of a high-quality single crystalline sample by electrical transport experiments. Our data show that the superconductor goes through a complex dimensional crossover below the onset Tc of 4.5 K. First, a quasi-1D fluctuating superconducting state with finite resistance forms in the CoC4 ribbons which are embedded in a Sc matrix in this material. At lower temperature, the transversal Josephson or proximity coupling of neighboring ribbons establishes a 3D bulk superconducting state. This dimensional crossover is very similar to Tl2Mo6Se6, which for a long time has been regarded as the most appropriate model system of a quasi-1D superconductor. Sc3CoC4 appears to be even more in the 1D limit than Tl2Mo6Se6.",1211.5430v4 2012-11-26,Local transport measurements at mesoscopic length scales using scanning tunneling potentiometry,"Under mesoscopic conditions, the transport potential on a thin film with current is theoretically expected to bear spatial variation due to quantum interference. Scanning tunneling potentiometry is the ideal tool to investigate such variation, by virtue of its high spatial resolution. We report in this {\it Letter} the first detailed measurement of transport potential under mesoscopic conditions. Epitaxial graphene at a temperature of 17K was chosen as the initial system for study because the characteristic transport length scales in this material are relatively large. Tip jumping artifacts are a major possible contribution to systematic errors; and we mitigate such problems by using custom-made slender and sharp tips manufactured by focussed ion beam. In our data, we observe residual resistivity dipoles associated with topoographical defects, and local peaks and dips in the potential that are not associated with topographical defects.",1211.6088v2 2012-12-06,Effects of spin density wave quantization on the electrical transport in epitaxial Cr thin films,"We present measurements of the electrical resistivity, $\rho$, in epitaxial Cr films of different thicknesses grown on MgO (100) substrates, as a function of temperature, $T$. The $\rho(T)$ curves display hysteretic behavior in certain temperature range, which is film thickness dependent. The hysteresis are related to the confinement of quantized incommensurate spin density waves (ISDW) in the film thickness. Our important finding is to experimentally show that the temperature $T_{mid}$ where the ISDW changes from $N$ to $N$\,+\,1 nodes {\it decreases} as the film thickness {\it increases}. Identifying $T_{mid}$ with a first order transition between ISDW states with $N$ and $N$\,+\,1 nodes, and using a Landau approach to the free energy of the ISDW together with Monte Carlo simulations, we show that the system at high temperatures explores all available modes for the ISDW, freezing out in one particular mode at a transition temperature that indeed decreases with film thickness, $L$. The detailed dependence of $T_{mid}(L)$ seems to depend rather strongly on the boundary conditions at the Cr film interfaces.",1212.1408v1 2013-01-09,Hall effect measurements on epitaxial SmNiO3 thin films and implications for antiferromagnetism,"The rare-earth nickelates (RNiO3) exhibit interesting phenomena such as unusual antiferromagnetic order at wavevector q = (1/2, 0, 1/2) and a tunable insulator-metal transition that are subjects of active research. Here we present temperature-dependent transport measurements of the resistivity, magnetoresistance, Seebeck coefficient, and Hall coefficient (RH) of epitaxial SmNiO3 thin films with varying oxygen stoichiometry. We find that from room temperature through the high temperature insulator-metal transition, the Hall coefficient is hole-like and the Seebeck coefficient is electron-like. At low temperature the N\'eel transition induces a crossover in the sign of RH to electron-like, similar to the effects of spin density wave formation in metallic systems but here arising in an insulating phase ~200 K below the insulator-metal transition. We propose that antiferromagnetism can be stabilized by bandstructure even in insulating phases of correlated oxides, such as RNiO3, that fall between the limits of strong and weak electron correlation.",1301.1968v3 2013-01-11,Batch-fabricated cantilever probes with electrical shielding for nanoscale dielectric and conductivity imaging,"This paper presents the design and fabrication of batch-processed cantilever probes with electrical shielding for scanning microwave impedance microscopy. The diameter of the tip apex, which defines the electrical resolution, is less than 50 nm. The width of the stripline and the thicknesses of the insulation dielectrics are optimized for a small series resistance (< 5 W) and a small background capacitance (~ 1 pF), both critical for high sensitivity imaging on various samples. The coaxial shielding ensures that only the probe tip interacts with the sample. The structure of the cantilever is designed to be symmetric to balance the stresses and thermal expansions of different layers so that the cantilever remains straight under variable temperatures. Such shielded cantilever probes produced in the wafer scale will facilitate enormous applications on nanoscale dielectric and conductivity imaging.",1301.2402v1 2013-01-14,Pressure-Induced Superconductivity and Its Scaling with Doping-Induced Superconductivity in the Iron Pnictide with Skutterudite Intermediary Layers,"The Ca10(PtnAs8)(Fe2As2)5 (n=3,4) compounds are a new type of iron pnictide superconductors whose structures consist of stacking Ca-PtnAs8-Ca-Fe2As2 layers in a unit cell. When n=3 (the 10-3-8 phase), the undoped compound is an antiferromagnetic (AFM) semiconductor, while, when n=4 (the 10-4-8 phase), the undoped compound is a superconductor with the transition temperature of 26K. Here we report the results of high-pressure studies on the 10-3-8 compound obtained through a combination of in-situ resistance, magnetic susceptibility, and Hall coefficient measurements. We find that its AFM order can be suppressed completely at 3.5 GPa and then superconducting state appears in the pressure range of 3.5-7 GPa. The pressure dependence of superconducting transition temperature displays a dome-like shape.",1301.2863v2 2013-02-08,Electrical transport across Au/Nb:SrTiO3 Schottky interface with different Nb doping,"We have investigated electron transport in Nb doped SrTiO$_3$ single crystals for two doping densities. We find that the resistivity and mobility are temperature dependent in both whereas the carrier concentration is almost temperature invariant. We rationalize this using the hydrogenic theory for shallow donors. Further, we probe electrical transport across Schottky interfaces of Au on TiO$_2$ terminated n-type SrTiO$_3$. Quantitative analysis of macroscopic I-V measurements reveal thermionic emission dominated transport for the low doped substrate whereas it deviates from such behavior for the high doped substrate. This work is relevant for designing devices to study electronic transport using oxide-semiconductors.",1302.2096v1 2013-02-14,Transport studies of dual-gated ABC and ABA trilayer graphene: band gap opening and band structure tuning in very large perpendicular electric field,"We report on the transport properties of ABC and ABA stacked trilayer graphene using dual, locally gated field effect devices. The high efficiency and large breakdown voltage of the HfO2 top and bottom gates enables independent tuning of the perpendicular electric field and the Fermi level over an unprecedentedly large range. We observe a resistance change of six orders of magnitude in the ABC trilayer, which demonstrates the opening of a band gap. Our data suggest that the gap saturates at a large displacement field of D ~ 3 V/nm, in agreement with self-consistent Hartree calculations. In contrast, the ABA trilayer remains metallic even under a large perpendicular electric field. Despite the absence of a band gap, the band structure of the ABA trilayer continues to evolve with increasing D. We observe signatures of two-band conduction at large D fields. Our self-consistent Hartree calculation reproduces many aspects of the experimental data, but also points to the need for more sophisticated theory.",1302.3432v1 2013-02-21,Superconductivity induced by U-doping in the SmFeAsO system,"Through partial substitution of Sm by U in SmFeAsO, a different member of the family of iron-based superconductors was successfully synthesized. X-ray diffraction measurements show that the lattice constants along the a and c axes are both squeezed through U doping, indicating a successful substitution of U at the Sm site. The parent compound shows a strong resistivity anomaly near 150 K, associated with spin-density-wave instability.U doping suppresses this instability and leads to a transition to the superconducting state at temperatures up to 49 K. Magnetic measurements confirm the bulk superconductivity in this system. For the sample with a doping level of x = 0.2, the external magnetic field suppresses the onset temperature very slowly, indicating a rather high upper critical field. In addition, the Hall effect measurements show that U clearly dopes electrons into the material.",1302.5155v1 2013-04-10,Pinning in a Porous Bi2223,"The current-voltage characteristics of a porous superconductor Bi2Sr2Ca2Cu3Ox (Bi2223) have been measured at temperature range from 10 to 90 K. The experimental dependences have been analyzed within the model allowing for pinning by clusters of a normal phase with fractal boundaries, as well as the model taking into account phase transformations of vortex matter. It has been found that the electrical resistance of the superconductor material significantly increases at temperatures of 60-70 K over the entire range of magnetic fields under consideration without changing in the sign of the curvature of the R(I) dependence. The melting of the vortex structure occurs at these temperatures. It has been assumed that this behavior is associated with the specific feature of the pinning in a highly porous high-temperature superconductor, which lies in the fractal distribution of pinning centers in a wide range of self-similarity scales.",1304.2844v1 2013-04-10,Multi-band superconductivity and nanoscale inhomogeneity at oxide interfaces,"The two-dimensional electron gas at the LaTiO3/SrTiO3 or LaAlO3/SrTiO3 oxide interfaces becomes superconducting when the carrier density is tuned by gating. The measured resistance and superfluid density reveal an inhomogeneous superconductivity resulting from percolation of filamentary structures of superconducting ""puddles"" with randomly distributed critical temperatures, embedded in a non-superconducting matrix. Following the evidence that superconductivity is related to the appearance of high-mobility carriers, we model intra-puddle superconductivity by a multi-band system within a weak coupling BCS scheme. The microscopic parameters, extracted by fitting the transport data with a percolative model, yield a consistent description of the dependence of the average intra-puddle critical temperature and superfluid density on the carrier density.",1304.2970v1 2013-04-22,Electrical transport in C-doped GaAs nanowires: surface effects,"The resistivity and the mobility of Carbon doped GaAs nanowires have been studied for different doping concentrations. Surface effects have been evaluated by comparing upassivated with passivated nanowires. We directly see the influence of the surface: the pinning of the Fermi level and the consequent existence of a depletion region lead to an increase of the mobility up to 30 cm^2/(V*s) for doping concentrations lower than 3*10^18 cm^-3. Electron beam induced current measurements show that the minority carrier diffusion path can be as high as 190 nm for passivated nanowires.",1304.5891v1 2013-05-23,Electronic origin of the orthorhombic Cmca structure in compressed elements and binary alloys,"Formation of the complex structure with 16 atoms in the orthorhombic cell, space group Cmca (Pearson symbol oC16) was experimentally found under high pressure in the alkali elements (K, Rb, Cs) and polyvalent elements of groups IV (Si, Ge) and V (Bi). Intermetallic phases with this structure form under pressure in binary Bi-based alloys (Bi-Sn, Bi-In, Bi-Pb). Stability of the Cmca - oC16 structure is analyzed within the nearly free-electron model in the frame of Fermi sphere - Brillouin zone interaction. A Brillouin-Jones zone formed by a group of strong diffraction reflections close to the Fermi sphere is the reason for reduction of crystal energy and stabilization of the structure. This zone corresponds well to the 4 valence electrons in Si and Ge and leads to assume a spd-hybridization for Bi. To explain the stabilization of this structure within the same model in alkali metals, that are monovalent at ambient conditions, a possibility of an overlap of the core and valence band electrons at strong compression is considered. The assumption of the increase in the number of valence electrons helps to understand sequences of complex structures in compressed alkali elements and unusual changes in their physical properties such as electrical resistance and superconductivity.",1305.5341v1 2013-05-29,Intrinsic and extrinsic origins of low-frequency noise in GaAs/AlGaAs Schottky-gated nanostructures,"We study low-frequency noise in current passing through quantum point contacts fabricated from several GaAs/AlGaAs heterostructures with different layer structures and fabrication processes. In contrast to previous reports, there is no gate-dependent random telegraph noise (RTN) originating from tunneling through a Schottky barrier in devices fabricated using the standard low-damage process. Gate-dependent RTN appears only in devices fabricated with a high-damage process that induces charge trap sites. We show that the insertion of AlAs/GaAs superlattices in the AlGaAs barrier helps to suppress trap formation. Our results enable the fabrication of damage-resistant and thus low-noise devices.",1305.6701v1 2013-06-29,Coexistence of Half-Metallic Itinerant Ferromagnetism with Local-Moment Antiferromagnetism in Ba{0.60}K{0.40}Mn2As2,"Magnetization, nuclear magnetic resonance, high-resolution x-ray diffraction and magnetic field-dependent neutron diffraction measurements reveal a novel magnetic ground state of Ba{0.60}K{0.40}Mn2As2 in which itinerant ferromagnetism (FM) below a Curie temperature TC = 100 K arising from the doped conduction holes coexists with collinear antiferromagnetism (AFM) of the Mn local moments that order below a Neel temperature TN = 480 K. The FM ordered moments are aligned in the tetragonal ab-plane and are orthogonal to the AFM-ordered Mn moments that are aligned along the c-axis. The magnitude and nature of the low-T FM ordered moment correspond to complete polarization of the doped-hole spins (half-metallic itinerant FM) as deduced from magnetization and ab-plane electrical resistivity measurements.",1307.0091v2 2013-07-22,Dimensional-Crossover-Driven Mott Insulators in SrVO3 Ultrathin Films,"High-quality epitaxial SrVO3 (SVO) thin films of various thicknesses were grown on (001)-oriented LSAT substrates by pulsed electron-beam deposition technique. Thick SVO films (~25 nm) exhibited metallic behavior with the electrical resistivity following the T2 law corresponding to a Fermi liquid system. We observed a temperature driven metal-insulator transition (MIT) in SVO ultrathin films with thicknesses below 6.5 nm, the transition temperature TMIT was found to be at 50 K for the 6.5 nm film, 120 K for the 5.7 nm film and 205 K for the 3 nm film. The emergence of the observed MIT can be attributed to the dimensional crossover from a three-dimensional metal to a two-dimensional Mott insulator, as the resulting reduction in the effective bandwidth W opens a band gap at the Fermi level. The magneto-transport study of the SVO ultrathin films also confirmed the observed MIT is due to the electron-electron interactions other than localization.",1307.5819v2 2013-07-26,Electron-phonon coupling in cuprate and iron-based superconductors revealed by Raman scattering,"Electron-phonon coupling (EPC) is one of the most common and fundamental interactions in solids. It not only dominates many basic dynamic processes like resistivity, thermal conductivity etc, but also provides the pairing glue in conventional superconductors. But in high-temperature superconductors (HTSC), it is still controversial whether or not EPC is in favor of paring. Despite the controversies, many experiments have provided clear evidence for EPC in HTSC. In this paper, we briefly review EPC in cuprate and iron-based superconducting systems revealed by Raman scattering. We introduce how to extract the coupling information through phonon lineshape. Then we discuss the strength of EPC in different HTSC systems and possible factors affecting the strength. The comparative study between Raman phonon theories and experiments allows us to gain insight into some crucial electronic properties, especially superconductivity. Finally we summarize and compare EPC in the two existing HTSC systems, and discuss what role it may play in HTSC.",1307.6972v1 2014-02-10,Evolution and defect analysis of vertical graphene nanosheets,"We report catalyst-free direct synthesis of vertical graphene nanosheets (VGNs) on SiO2/Si and quartz substrates using microwave electron cyclotron resonance - plasma enhanced chemical vapor deposition. The evolution of VGNs is studied systematically at different growth stages. Raman analysis as a function of growth time reveals that two different disorder-induced competing mechanisms contributing to the defect band intensity. The VGNs grown on SiO2/Si substrates predominantly consists of both vacancy-like and hopping defects. On the other hand, the VGNs grown on quartz substrates contain mainly boundary-like defects. XPS studies also corroborate Raman analysis in terms of defect density and vacancy-like defects for the VGNs grown on SiO2/Si substrates. Moreover, the grown VGNs exhibit a high optical transmittance from 95 to 78 % at 550 nm and the sheet resistance varies from 30 to 2.17 kohms/square depending on growth time.",1402.2074v3 2014-02-19,Phase Diagram of Micron-Size Bridges of SrTiO$_3/$LaAlO$_3$ Interface: Link Between Multiple Band Structure and Superconductivity,"The rich phase diagram of the two dimensional electron gas (2DEG) at the \STO/\LAO interface is probed using Hall and longitudinal resistivity. Thanks to a special bridge design we are able to tune through the superconducting transition temperature T$_c$ and to mute superconductivity by either adding or removing carriers in a gate bias range of a few volts. Hall signal measurements pinpoint the onset of population of a second mobile band right at the carrier concentration where maximum superconducting T$_c$ and critical field H$_c$ occur. These results emphasize the advantages of our design, which can be applied to many other two dimensional systems assembled on top of a dielectric substrate with high permittivity.",1402.4646v1 2014-03-04,Effect of modulations of doping and strain on the electron transport in monolayer MoS_2,"The doping and strain effects on the electron transport of monolayer MoS_2 are systematically investigated using the first-principles calculations with Boltzmann transport theory. We estimate the mobility has a maximum 275 cm^2/(Vs) in the low doping level under the strain-free condition. The applying a small strain (3%) can improve the maximum mobility to 1150 cm^2/(Vs) and the strain effect is more significant in the high doping level. We demonstrate that the electric resistance mainly due to the electron transition between K and Q valleys scattered by the M momentum phonons. However, the strain can effectively suppress this type of electron-phonon coupling by changing the energy difference between the K and Q valleys. This sensitivity of mobility to the external strain may direct the improving electron transport of MoS_2.",1403.0695v2 2014-03-29,Two components for one resistivity in LaVO3/SrTiO3 heterostructures,"A series of 100 nm LaVO3 thin films have been synthesized on (001)-oriented SrTiO3 substrates using the pulsed laser deposition technique, and the effects of growth temperature are analyzed. Transport properties reveal a large electronic mobility and a non-linear Hall effect at low temperature. In addition, a cross-over from a semiconducting state at high-temperature to a metallic state at low-temperature is observed, with a clear enhancement of the metallic character as the growth temperature increases. Optical absorption measurements combined with the two-bands analysis of the Hall effect show that the metallicity is induced by the diffusion of oxygen vacancies in the SrTiO3 substrate. These results allow to understand that the film/substrate heterostructure behaves as an original semiconducting-metallic parallel resistor, and electronic transport properties are consistently explained.",1403.7648v2 2014-04-07,Directional pinning and anisotropy in YBa2Cu3O7-x with BaZrO3 nanorods: intrinsic and nanorods-induced anisotropy,"We present a study of the anisotropic vortex parameters as obtained from measurements of the microwave complex resistivity in the vortex state with a tilted applied magnetic field in YBa2Cu3O7-x thin films with BaZrO3 nanorods. We present the angular dependence of the vortex viscosity $\eta$, the pinning constant k_p and the upper limit for the creep factor \chi_M. We show that the directional effect of the nanorods is absent in \eta, which is dictated by the mass anisotropy \gamma. By contrast, pinning-mediated properties are strongly affected by the nanorods. It is significant that the pinning and creep affected by the nanorods is detectable also at our very high operating frequency, which implies very short-range displacements of the vortices from their equilibrium position.",1404.1670v1 2014-05-07,Anisotropic giant magnetoresistance in NbSb2,"The extremely large transverse magnetoreistance (the magnetoresistant ratio $\sim 1.3\times10^5\%$ in 2 K and 9 T field, and $4.3\times 10^6\%$ in 0.4 K and 32 T field, without saturation), and the metal-semiconductor crossover induced by magnetic field, are reported in NbSb$_2$ single crystal with electric current parallel to the $b$-axis. The metal-semiconductor crossover is preserved when the current is along the $ac$-plane but the magnetoresistant ratio is significantly suppressed. The sign reversal of the Hall resistivity in the field close to the crossover point, and the electronic structure calculation reveals the coexistence of a small number of holes with very high mobility and a large number of electrons with low mobility. These effects are attributed to the change of the Fermi surface induced by the magnetic field.",1405.1719v2 2014-06-05,Current transport and thermoelectric properties of very high power factor Fe3O4 / SiO2 / p-type Si (001) devices,"The current transport and thermoelectric properties of Fe3O4 / SiO2 / p-type Si(001) heterostructures with Fe3O4 thicknesses of 150, 200, and 350 nm have been investigated between 100 and 300 K. We observe a sharp drop of the in-plane resistivity at 200K due to the onset of conduction along the Si / SiO2 interface related to tunneling of electrons from the Fe3O4 into the accumulation layer of holes at the Si / SiO2 interface, whose existence was confirmed by capacitance-voltage measurements and a two band analysis of the Hall effect. This is accompanied by a large increase of the Seebeck coefficient reaching +1000 {\mu}V/K at 300K that is related to holes in the p-type Si(001) and gives a power factor of 70 mW/K2m when the Fe3O4 layer thickness is reduced down to 150 nm. We show that most of the current flows in the Fe3O4 layer at 300 K, while the Fe3O4 / SiO2 / p-type Si(001) heterostructures behave like tunneling p-n junctions in the transverse direction.",1406.1282v1 2014-06-20,Anomalous Hall Effect in Ge(1-x-y)Pb(x)Mn(y)Te Composite System,"The purpose of this study was to investigate the magnetotransport properties of the Ge(0.743)Pb(0.183)Mn(0.074)Te mixed crystal. The results of magnetization measurements indicated that the compound is a spin-glass-like diluted magnetic semiconductor with critical temperature TSG = 97.5 K. Nanoclusters in the sample are observed. Both, matrix and clusters are magnetically active. Resistivity as a function of temperature has a minimum at 30 K. Below the minimum a variable-range hopping is observed, while above the minimum a metallic-like behavior occurs. The crystal has high hole concentration, p = 6.6E20 cm-3, temperature-independent. Magnetoresistance amplitude changes from -0.78 to 1.18% with increase of temperature. In the magnetotransport measurements we observed the anomalous Hall effect (AHE) with hysteresis loops. Calculated AHE coefficient, RS = 2.0E6 m3/C, is temperature independent. The analysis indicates the extrinsic skew scattering mechanism to be the main physical mechanism responsible for AHE in Ge(0.743)Pb(0.183)Mn(0.074)Te alloy.",1406.5294v1 2014-07-22,Universal scaling of the critical temperature for thin films near the superconducting-to-insulating transition,"Thin superconducting films form a unique platform for geometrically-confined, strongly-interacting electrons. They allow an inherent competition between disorder and superconductivity, which in turn enables the intriguing superconducting-to-insulator transition and believed to facilitate the comprehension of high-Tc superconductivity. Furthermore, understanding thin film superconductivity is technologically essential e.g. for photo-detectors, and quantum-computers. Consequently, the absence of an established universal relationships between critical temperature ($T_c$), film thickness ($d$) and sheet resistance ($R_s$) hinders both our understanding of the onset of the superconductivity and the development of miniaturised superconducting devices. We report that in thin films, superconductivity scales as $d^.$$T_c(R_s)$. We demonstrated this scaling by analysing the data published over the past 46 years for different materials (and facilitated this database for further analysis). Moreover, we experimentally confirmed the discovered scaling for NbN films, quantified it with a power law, explored its possible origin and demonstrated its usefulness for superconducting film-based devices.",1407.5945v2 2014-09-18,Electrical and optical properties of ITO thin films prepared by DC magnetron sputtering for low-emitting coatings,"Optimized DC magnetron sputtering system for the deposition of transparent conductive oxides (TCOs), such indium tin oxide (ITO) on glass substrate has been applied in order to achieve low-emitting (low-e) transparent coatings. To obtain the concerned electrical resistance and high infrared reflection, first the effect of applied sputtering power then oxygen flow on the properties of films have been investigated. The other depositions parameters are kept constant. Film deposition at at temperature 400 degree of Celsius in oxygen flow of 3 Standard Cubic Centimeters per Minute results in transparent and infrared reflecting coatings. Under this condition the highest attained average reflectance in the infrared is ({\lambda}=3-25 micron) 89.5% (lowest emittance equals to less than 11%), whereas transparency in the visible is 85% approximately. Plasma wavelength and carrier concentration was measured.",1409.5293v1 2014-09-25,Characterisation of Glass Electrodes and RPC Detectors for $INO-ICAL$ Experiment,"India-based Neutrino Observatory (INO) is a planned neutrino experiment to be build up in southern part of India.The INO observatory will host a 51 kton Iron Calorimeter (ICAL) detector to detect atmospheric neutrinos. Resistive Plate Chamber (RPC) has been chosen as the active detector element for the ICAL experiment. The ICAL experiment will consist of about 28,000 RPC's of dimension $2~m\times 2~m$, divided into three modules. The experiment is planned to take data at least for 20 years from its start date. Due to the large number of RPC needed for ICAL experiment and the long lifetime of the experiment, it is necessary to carry out detailed $R\&D$ to optimise each and every parameter of the detector performance. We report on the performance studies carried out on the RPC's made with these electrodes, and finally compare the detector performance with that of the material properties to optimise the detector parameters.",1409.7184v1 2014-11-24,Thermoelectric power of bulk black-phosphorus,"The potential of bulk black-phosphorus for thermoelectric applications has been experimentally studied. The Seebeck Coefficient (S) has been measured in the temperature range from 300 K to 385 K, finding a value of S = +335 +- 10 uV/K at room temperature (indicating a naturally occurring p-type conductivity). S increases with temperature, as expected for p-type semiconductors, which can be attributed to an increase of the charge carrier density. The electrical resistance drops up to a 40 % while heating in the studied temperature range. As a consequence, the power factor at 385 K is 2.7 times higher than that at room temperature. This work demonstrates the feasibility of black-phosphorus in thermoelectric applications, such as thermal energy scavenging, which typically require devices with high performance at temperatures above room temperature.",1411.6468v2 2014-11-26,Towards high mobility InSb nanowire devices,"We study the low-temperature electron mobility of InSb nanowires. We extract the mobility at 4.2 Kelvin by means of field effect transport measurements using a model consisting of a nanowire-transistor with contact resistances. This model enables an accurate extraction of device parameters, thereby allowing for a systematic study of the nanowire mobility. We identify factors affecting the mobility, and after optimization obtain a field effect mobility of $\sim2.5\mathbin{\times}10^4$ cm$^2$/Vs. We further demonstrate the reproducibility of these mobility values which are among the highest reported for nanowires. Our investigations indicate that the mobility is currently limited by adsorption of molecules to the nanowire surface and/or the substrate.",1411.7285v2 2014-12-22,Large anisotropic thermal conductivity of intrinsically two-dimensional metallic oxide PdCoO$_2$,"The highly conductive layered metallic oxide \pdcoo{} is a near-perfect analogue to an alkali metal in two dimensions. It is distinguished from other two-dimensional electron systems where the Fermi surface does not reach the Brillouin zone boundary by a high planar electron density exceeding $10^{15}$ cm$^{-2}$. The simple single-band quasi-2D electronic structure results in strongly anisotropic transport properties and limits the effectiveness of electron-phonon scattering. Measurements on single crystals in the temperature range from 10-300K show that the thermal conductivity is much more weakly anisotropic than the electrical resistivity, as a result of significant phonon heat transport. The in-plane thermoelectric power is linear in temperature at 300\,K and displays a purity-dependent peak around 50K. Given the extreme simplicity of the band-structure, it is possible to identify this peak with phonon drag driven by normal electron-phonon scattering processes.",1412.6919v1 2015-02-06,Anomalous Pressure Dependence of magnetic Ordering Temperature in Tb to 141 GPa: Comparison with Gd and Dy,"In previous studies the pressure dependence of the magnetic ordering temperature $T_{\text{o}}$ of Dy was found to exhibit a sharp increase above its volume collapse pressure of 73 GPa, appearing to reach temperatures well above ambient at 157 GPa. In a search for a second such lanthanide, electrical resistivity measurements were carried out on neighboring Tb to 141 GPa over the temperature range 3.8 - 295 K. Below Tb's volume collapse pressure of 53 GPa, the pressure dependence $T_{\text{o}}(P)$ mirrors that of both Dy and Gd. However, at higher pressures $T_{\text{o}}(P)$ for Tb becomes highly anomalous. This result, together with the very strong suppression of superconductivity by dilute Tb ions in Y, suggests that extreme pressure transports Tb into an unconventional magnetic state with an anomalously high magnetic ordering temperature.",1502.01785v1 2015-02-07,Interband Tunneling for Hole Injection in III-Nitride Ultra-violet Emitters,"Ultra-violet emitters have several applications in the areas of sensing, water purification, and data storage. While the III-Nitride semiconductor system has the band gap region necessary for ultraviolet emission, achieving efficient ultraviolet solid state emitters remains a challenge due to the low p-type conductivity and high contact resistance in wide band gap AlGaN-based ultra-violet light emitters. In this work, we show that efficient interband tunneling can be used for non-equilibrium injection of holes into ultraviolet emitters. Polarization-engineered tunnel junctions were used to enhance tunneling probability by several orders of magnitude over a PN homojunction, leading to highly efficient tunnel injection of holes to ultraviolet light emitters. This demonstration of efficient interband tunneling introduces a new paradigm for design of ultra-violet light emitting diodes and diode lasers, and enables higher efficiency and lower cost ultra-violet emitters.",1502.02080v1 2015-02-27,"Quantum oscillations, thermoelectric coefficients and the Fermi surface of semi-metallic WTe2","We present a study of angle-resolved quantum oscillations of electric and thermoelectric transport coefficients in semi-metallic WTe$_{2}$, which has the particularity of displaying a large B$^{2}$ magneto-resistance. The Fermi surface consists of two pairs of electron-like and hole-like pockets of equal volumes in a ""Russian doll"" structure. Carrier density, Fermi energy, mobility and the mean-free-path of the system are quantified. An additional frequency is observed above a threshold field and attributed to magnetic breakdown across two orbits. In contrast to all other dilute metals, the Nernst signal remains linear in magnetic field even in the high-field ($\omega_c\tau \gg 1$) regime. Surprisingly, none of the pockets extend across the c-axis of the first Brillouin zone, making the system a three-dimensional metal with moderate anisotropy in Fermi velocity yet a large anisotropy in mean-free-path.",1502.07797v2 2015-05-19,Energy Exchange between Phononic and Electronic Subsystem Governing The Nonlinear Conduction in DCNQI$_2$Cu,"We present a dynamical study on the nonlinear conduction behaviour in the commensurate charge-density-wave phase of the quasi-one-dimensional conductor DCNQI$_2$Cu below 75 K. We can accurately simulate magnitude and time-dependence of the measured conductivity in response to large voltage pulses by accounting for the energy exchange between the phononic and electronic subsystems by means of an electrothermal model. Our simulations reveal a distinct non-equilibrium population of optical phonon states with an average energy of E$_{ph}$ = 19 meV being half the activation energy of about $\Delta$E$_a$ = 39 meV observed in DC resistivity measurements. By inelastic scattering, this hot optical phonon bath generates additional charge-carrying excitations thus providing a multiplication effect while energy transferred to the acoustic phonons is dissipated out of the system via heat conduction. Therefore, in high electric fields a preferred interaction of charge-carrying excitations with optical phonons compared to acoustic phonon modes is considered to be responsible for the nonlinear conduction effects observed in DCNQI$_2$Cu.",1505.04907v2 2015-08-19,Argument on superconductivity pairing mechanism from cobalt impurity doping in FeSe: spin ($s_{\pm}$) or orbital ($s_{++}$) fluctuation,"In high-superconducting transition temperature ($T_{\rm c}$) iron-based superconductors, interband sign reversal ($s_{\rm \pm}$) and sign preserving ($s_{\rm ++}$) $s$-wave superconducting states have been primarily discussed as the plausible superconducting mechanism. We study Co impurity scattering effects on the superconductivity in order to achieve an important clue on the pairing mechanism using single crystal Fe$_{1-x}$Co$_x$Se and depict a phase diagram of a FeSe system. Both superconductivity and structural transition / orbital order are suppressed by the Co replacement on the Fe sites and disappear above $x$ = 0.036. These correlated suppressions represent a common background physics behind these physical phenomena in the multiband Fermi surfaces of FeSe. By comparing experimental data and theories so far proposed, the suppression of $T_{\rm c}$ against the residual resistivity is shown to be much weaker than that predicted in the case of a general sign reversal and a full gap $s_{\pm}$ models. The origin of the superconducting paring in FeSe is discussed in terms of its multiband electronic structure.",1508.04605v2 2015-08-19,Electric field control of spin lifetimes in Nb-SrTiO$_3$ by spin-orbit fields,"We show electric field control of the spin accumulation at the interface of the oxide semiconductor Nb-SrTiO$_{3}$ with Co/AlO$_{x}$ spin injection contacts at room temperature. The in-plane spin lifetime $\tau_\parallel$ as well as the ratio of the out-of-plane to in-plane spin lifetime $\tau_\perp/\tau_\parallel$ is manipulated by the built-in electric field at the semiconductor surface, without any additional gate contact. The origin of this manipulation is attributed to Rashba Spin-Orbit Fields (SOFs) at the Nb-SrTiO$_3$ surface and shown to be consistent with theoretical model calculations based on SOF spin flip scattering. Additionally, the junction can be set in a high or low resistance state, leading to a non-volatile control of $\tau_\perp/\tau_\parallel$, consistent with the manipulation of the Rashba SOF strength. Such room temperature electric field control over the spin state is essential for developing energy-efficient spintronic devices and shows promise for complex oxide based (spin)electronics",1508.04649v1 2015-09-13,Effects of Cr substitution on the magnetic and transport properties and electronic states of SrRuO3 epitaxial thin films,"The effect of Cr substitution in a SrRuO3 epitaxial thin film on SrTiO3 substrate was investigated by measuring the magnetic and transport properties and the electronic states. The ferromagnetic transition temperature of the SrRu0.9Cr0.1O3 film (166 K) was higher than that of the SrRuO3 film (147 K). Resonant photoemission spectroscopy experimentally revealed that the Cr 3dt2g orbital is hybridized with the Ru 4dt2g orbital in the SrRu0.9Cr0.1O3 film, supporting the assumption that the enhancement of the ferromagnetic transition temperature through Cr substitution stems from the widening of energy bands due to the hybridization of Cr 3dt2g and Ru 4dt2g orbitals. Furthermore, we found that the Hall resistivity of the SrRu0.9Cr0.1O3 film at low temperature is not a linear function of magnetic field in the high-field region where the out-of-plane magnetization was saturated; this result suggests that the SrRu0.9Cr0.1O3 film undergoes a structural transition at low temperature accompanied with the modulation of the Fermi surface.",1509.03804v1 2015-10-22,Anomalous transport and thermoelectric performances of CuAgSe compounds,"The copper silver selenide has two phases: the low-temperature semimetal phase ({\alpha}-CuAgSe) and high-temperature phonon-glass superionic phase (\b{eta}-CuAgSe). In this work, the electric transport and thermoelectric properties of the two phases are investigated. It is revealed that the \b{eta}-CuAgSe is a p-type semiconductor and exhibits low thermal conductivity while the {\alpha}-CuAgSe shows metallic conduction with dominant n-type carriers and low electrical resistivity. The thermoelectric figure of merit zT of the polycrystalline \b{eta}-CuAgSe at 623 K is ~0.95, suggesting that superionic CuAgSe can be a promising thermoelectric candidate in the intermediate temperature range.",1510.06616v1 2015-11-12,Experimental and numerical analysis of tribological behavior of CrAl(Si)N films during Scratch,"Scratch sliding tests with a ZrO2 ball and CrAlSiN films with different Si content were conducted due to CrAlSiN films having high hardness and good wear resistance. After up to 6000 cycles the specimens were analyzed by Scanning Electron Microscopy. The friction coefficient of CrAlSiN was lower than that of CrAlN film.A corresponding three-dimensional finite element model was constructed with the help of the ABAQUS to describe the mechanical response during scratch. A comparison of experimental and computational results revealed that the small elastic deformation took place in the films and substrates;the deformation friction coefficient was negligible in comparison with the Coulomb friction coefficient;and with increasing Young's modulus, the stress concentration was more obvious in CrAlSiN than in CrAlN.",1511.04092v2 2015-12-27,Room-temperature paramagnetoelectric effect in magnetoelectric multiferroics Pb(Fe1/2Nb1/2)O3 and its solid solution with PbTiO3,"We have observed the magnetoelectric response at room temperature and above in high-resistive ceramics made of multiferroic Pb(Fe1/2Nb1/2)O3 (PFN) and PFN-based solid solution 0.91PFN-0.09PbTiO3 (PFN-PT). The value of the paramagnetoelectric (PME) coefficient shows a pronounced maximum near the ferroelectric-to-paraelectric phase transition temperature, T_C, and then decreases sharply to zero for T>T_C. The maximal PME coefficient in PFN is about 4x10(-18) s/A. The theoretical description of the PME effect, within the framework of a Landau theory of phase transitions allowing for realistic temperature dependences of spontaneous polarization, dielectric and magnetic susceptibilities, qualitatively reproduces well the temperature dependence of the PME coefficient. In particular, the Landau theory predicts the significant increase of the PME effect at low temperatures and near the temperature of the paraelectric-to-ferroelectric phase transition, since the PME coefficient is equal to the product of the spontaneous polarization, dielectric permittivity, square of magnetic susceptibility and the coefficient quantifying the strength of the biquadratic magnetoelectric coupling",1512.08217v1 2015-12-31,Intrinsic Nanotwin Effect on Thermal Boundary Conductance in Bulk and Single-Nanowire Twinning Superlattices,"Coherent twin boundaries form periodic lamellar twinning in a wide variety of semiconductor nanowires, and are often viewed as near-perfect interfaces with reduced phonon and electron scattering behaviors. Such unique characteristics are of practical interest for high-performance thermoelectrics and optoelectronics; however, insufficient understanding of twin-size effects on thermal boundary resistance poses significant limitations for potential applications. Here, using atomistic simulations and ab-initio calculations, we report direct computational observations showing a crossover from diffuse interface scattering to superlattice-like behavior for thermal transport across nanoscale twin boundaries present in prototypical bulk and nanowire Si examples. Intrinsic interface scattering is identified for twin periods larger than or equal to 22.6 nm, but also vanishes below this size to be replaced by ultrahigh Kapitza thermal conductances. Detailed analysis of vibrational modes shows that modeling twin boundaries as atomically-thin 6H-Si layers, rather than phonon scattering interfaces, provides an accurate description of effective cross-plane and in-plane thermal conductivities in twinning superlattices, as a function of the twin period thickness.",1512.09357v2 2016-02-20,Investigation of the electron-phonon interaction in $N{{b}_{3}}Sn$ with the aid of microcontacts,"The method of microcontact spectroscopy in the superconducting state was used to investigate weak nonlinearities of the current-voltage characteristics of point contacts made of $N{{b}_{3}}Sn$ single crystals. The nature of the spectrum of the electron-phonon interaction was found to vary considerably from contact to contact, indicating considerable deviations of the composition of the surface of $N{{b}_{3}}Sn$ from stoichiometry. A correlation was established between the nature of the spectrum and the magnitude of the gap singularities of the current-voltage characteristics. In the case of ""dirty"" high-resistance contacts with strong gap singularities the microcontact spectra were reasonably reproducible, which made it possible to relate them sufficiently closely to the microcontact function of the electron-phonon interaction in the bulk material. It was found that microcontact spectroscopy of this interaction was possible in the superconducting state not only in dirty $S-c-S$ contacts, but also in dirty $S-c-N$ contacts.",1602.06398v1 2016-04-11,"Single crystal growth of CeTAl$_3$ (T = Cu, Ag, Au, Pd and Pt)","We report single crystal growth of the series of CeTAl$_3$ compounds with T = Cu, Ag, Au, Pd and Pt by means of optical float zoning. High crystalline quality was confirmed in a thorough characterization process. With the exception of CeAgAl$_3$, all compounds crystallize in the non-centrosymmetric tetragonal BaNiSn$_{3}$ structure (space group: I4mm, No. 107), whereas CeAgAl$_3$ adopts the related orthorhombic PbSbO$_2$Cl structure (Cmcm, No. 63). An attempt to grow CeNiAl$_3$ resulted in the composition CeNi$_2$Al$_5$. Low temperature resistivity measurements down to $\sim$0.1K did not reveal evidence suggestive of magnetic order in CePtAl$_3$ and CePdAl$_3$. In contrast, CeAuAl$_3$, CeCuAl$_3$ and CeAgAl$_3$ display signatures of magnetic transitions at 1.3K, 2.1K and 3.2K, respectively. This is consistent with previous reports of antiferromagnetic order in CeAuAl$_3$, and CeCuAl$_3$ as well as ferromagnetism in CeAgAl$_3$, respectively.",1604.03146v1 2016-04-14,Large magnetothermopower and Fermi surface reconstruction in Sb$_2$Te$_2$Se,"We report the magnetoresistance, magnetothermopower and quantum oscillation study of Sb$_2$Te$_2$Se single crystal. The in-plane transverse magnetoresistance exhibits a crossover at a critical field $B^*$ from semiclassical weak-field $B^2$ dependence to the high-field unsaturated linear magnetoresistance which persists up to the room temperature. The low-temperature Seebeck coefficient is negative in zero field contrary to the positive Hall resistivity, indicating the multiband effect. The magnetic field induced the sign reversion of the Seebeck coefficient between 2 K and 150 K, . The quantum oscillation of crystals reveals the quasi-two-dimensional (quasi-2D) Fermi surface. These effects are possibly attributed to the large Fermi surface which touches Brillouin zone boundary to becomes quasi-2D and the variation in the chemical potential induced by the magnetic field.",1604.04281v1 2016-04-15,Electronic Structure Descriptor for Discovery of Narrow-Band Red-Emitting Phosphors,"Narrow-band red-emitting phosphors are a critical component in phosphor-converted light-emitting diodes for highly efficient illumination-grade lighting. In this work, we report the discovery of a quantitative descriptor for narrow-band Eu2+-activated emission identified through a comparison of the electronic structure of known narrow-band and broad-band phosphors. We find that a narrow emission bandwidth is characterized by a large splitting of more than 0.1 eV between the two highest Eu2+ 4f7 bands. By incorporating this descriptor in a high throughput first principles screening of 2,259 nitride compounds, we identify five promising new nitride hosts for Eu2+-activated red-emitting phosphors that are predicted to exhibit good chemical stability, thermal quenching resistance and quantum efficiency, as well as narrow-band emission. Our findings provide important insights into the emission characteristics of rare-earth activators in phosphor hosts, and a general strategy to the discovery of phosphors with a desired emission peak and bandwidth.",1604.04581v1 2016-04-18,Superconductivity in undoped CaFe2As2 single crystals,"Single crystals of undoped CaFe2As2 were grown by a FeAs self-flux method, and the crystals were quenched in ice-water rapidly after high temperature growth. The quenched crystal undergoes a collapsed tetragonal structural phase transition around 80 K revealed by the temperature dependent X-ray diffraction measurements. Superconductivity below 25 K was observed in the collapsed phase by resistivity and magnetization measurements. The isothermal magnetization curve measured at 2 K indicates that this is a typical type-II superconductor. For comparison, we systematically characterized the properties of the furnace cooled, quenched, and post-annealed single crystals, and found strong internal crystallographic strain existing in the quenched samples, which is the key for the occurrence of superconductivity in the undoped CaFe2As2 single crystals.",1604.04964v1 2016-04-22,Multiband behavior and non-metallic low-temperature state of K$_{0.50}$Na$_{0.24}$Fe$_{1.52}$Se$_{2}$,"We report evidence for multiband transport and an insulating low-temperature normal state in superconducting K$_{0.50}$Na$_{0.24}$Fe$_{1.52}$Se$_{2}$ with $T_{c}\approx 20$ K. The temperature-dependent upper critical field, $H_{c2}$, is well described by a two-band BCS model. The normal-state resistance, accessible at low temperatures only in pulsed magnetic fields, shows an insulating logarithmic temperature dependence as $T \rightarrow 0$ after superconductivity is suppressed. This is similar as for high-$T_{c}$ copper oxides and granular type-I superconductors, suggesting that the superconductor-insulator transition observed in high magnetic fields is related to intrinsic nanoscale phase separation.",1604.06793v1 2016-05-30,High-field electron transport in bulk ZnO,"Current-voltage dependence is measured in (Ga,Sb)-doped ZnO up to 150 kV/cm electric fields. A channel temperature is controlled by applying relatively short (few ns) voltage pulses to two-terminal samples. The dependence of electron drift velocity on electron density ranging from 1.42$\times$10$^{17}$ cm$^{-3}$ to 1.3$\times$10$^{20}$ cm$^{-3}$ at a given electric field is deduced after estimation of the sample contact resistance and the Hall electron mobility. Manifestation of the highest electron drift velocity up to $\sim$1.5$\times$10$^{7}$ cm/s is estimated for electron density of 1.42$\times$10$^{17}$ cm$^{-3}$ and is in agreement with Monte Carlo simulation when hot-phonon lifetime is below 1 ps. A local drift velocity maximum is observed at $\sim$1.1$\times$10$^{19}$ cm$^{-3}$ and is in agreement with ultra-fast hot phonon decay.",1605.09117v1 2016-06-27,Hafnium carbide formation in oxygen deficient hafnium oxide thin films,"On highly oxygen deficient thin films of hafnium oxide (hafnia, HfO$_{2-x}$) contaminated with adsorbates of carbon oxides, the formation of hafnium carbide (HfC$_x$) at the surface during vacuum annealing at temperatures as low as 600 {\deg}C is reported. Using X-ray photoelectron spectroscopy the evolution of the HfC$_x$ surface layer related to a transformation from insulating into metallic state is monitored in situ. In contrast, for fully stoichiometric HfO$_2$ thin films prepared and measured under identical conditions, the formation of HfC$_x$ was not detectable suggesting that the enhanced adsorption of carbon oxides on oxygen deficient films provides a carbon source for the carbide formation. This shows that a high concentration of oxygen vacancies in carbon contaminated hafnia lowers considerably the formation energy of hafnium carbide. Thus, the presence of a sufficient amount of residual carbon in resistive random access memory devices might lead to a similar carbide formation within the conducting filaments due to Joule heating.",1606.08227v1 2016-06-29,Improved model for the thermal conductivity of binary metallic systems,"We extended and corrected Mott's two-band model for the composition-dependence of thermal and electrical conductivity in binary metal alloys based on high-throughput time-domain thermoreflectance (TDTR) measurements on diffusion multiples and scatterer-density calculations from first principles. Examining PdAg, PtRh, AuAg, AuCu, PdCu, PdPt, and NiRh binary alloys, we found that the nature of the two dominant scatterer-bands considered in the Mott model changes with the alloys, and should be interpreted as a combination of the dominant element-specific s- and/or d-orbitals. Using calculated orbital and element-resolved density-of-states values calculated with density functional theory as input, we determined the correct orbital mix that dominates electron scattering for all examined alloys and find excellent agreement between fitted models and experiments. The proposed description of the composition dependence of the resistivity can be readily implemented into the CALPHAD framework.",1606.09287v2 2016-06-30,Superconductivity at 5.5 K in Nb2PdSe5 compound,"We report superconductivity in as synthesized Nb2PdSe5, which is similar to recently discovered Nb2PdS5 compound having very high upper critical field, clearly above the Pauli paramagnetic limit [Sci. Rep. 3, 1446 (2013)]. A bulk polycrystalline Nb2PdSe5 sample is synthesized by solid state reaction route in phase pure structure. The structural characterization has been done by X ray diffraction, followed by Rietveld refinements, which revealed that Nb2PdSe5 sample is crystallized in monoclinic structure with in space group C2/m. Structural analysis revealed the formation of sharing of one dimensional PdSe2 chains. Electrical and magnetic measurements confirmed superconductivity in Nb2PdSe5 compound at 5.5K. Detailed magneto-resistance results, exhibited the value of upper critical field to be around 8.2Tesla. The estimated Hc2(0) is within Pauli Paramagnetic limit, which is unlike the Nb2PdS5.",1606.09369v2 2016-08-01,Phase Transition in IrTe$_2$ induced by spin-orbit coupling,"IrTe$_2$ has been renewed as an interesting system showing competing phenomenon between a questionable density-wave transition near 270 K followed by superconductivity with doping of high atomic number materials. Higher atomic numbers of Te and Ir supports strong spin-orbital coupling in this system. Using dynamical mean field theory with LDA band structure I have introduced Rashba spin orbit coupling in this system to get the interpretation for anomalous resistivity and related transition in this system. While no considerable changes are observed in DMFT results of Ir-5d band other than orbital selective pseudogap pinned to Fermi level, Te-p band shows a van Hove singularity at the Fermi level except low temperature. Finally I discuss the implications of these results in theoretical understanding of ordering in IrTe$_2$.",1608.00467v1 2016-08-03,Edge-induced Schottky barrier modulation at metal contacts to exfoliated molybdenum disulfide flakes,"Ultrathin two-dimensional semiconductors obtained from layered transition-metal dichalcogenides such as molybdenum disulfide (MoS2) are promising for ultimately scaled transistors beyond Si. Although the shortening of the semiconductor channel is widely studied, the narrowing of the channel, which should also be important for scaling down the transistor, has been examined to a lesser degree thus far. In this study, the impact of narrowing on mechanically exfoliated MoS2 flakes was investigated according to the channel-width-dependent Schottky barrier heights at Cr/Au contacts. Narrower channels were found to possess a higher Schottky barrier height, which is ascribed to the edge-induced band bending in MoS2. The higher barrier heights degrade the transistor performance as a higher electrode-contact resistance. Theoretical analyses based on Poisson's equation showed that the edge-induced effect can be alleviated by a high dopant impurity concentration, but this strategy should be limited to channel widths of roughly 0.7 micrometers because of the impurity-induced charge-carrier mobility degradation. Therefore, proper termination of the dangling bonds at the edges should be necessary for aggressive scaling with layered semiconductors.",1608.01061v1 2016-08-23,Chiral anomaly and longitudinal magnetotransport in type-II Weyl semimetals,"In the presence of parallel electric and magnetic fields, the violation of separate number conservation laws for the three dimensional left and right handed Weyl fermions is known as the chiral anomaly. The recent discovery of Weyl and Dirac semimetals has paved the way for experimentally testing the effects of chiral anomaly via longitudinal magneto-transport measurements. More recently, a type-II Weyl semimetal (WSM) phase has been proposed, where the nodal points possess a finite density of states due to the touching between electron- and hole- pockets. It has been suggested that the main difference between the two types of WSMs (type-I and type-II) is that in the latter, chiral anomaly and the associated longitudinal magneto-resistance are strongly anisotropic, vanishing when the applied magnetic field is perpendicular to the direction of tilt of Weyl fermion cones in a type-II WSM. We analyze chiral anomaly in a type-II WSM in quasiclassical Boltzmann framework, and find that the chiral anomaly induced positive longitudinal magneto-conductivity is present along any arbitrary direction.",1608.06625v2 2016-10-19,Anomalous Thermal Diffusivity in Underdoped YBa$_2$Cu$_3$O$_{6+x}$,"We present local optical measurements of thermal diffusivity in the $ab$ plane of underdoped YBCO crystals. We find that the diffusivity anisotropy is comparable to reported values of the electrical resistivity anisotropy, suggesting that the anisotropies have the same origin. The anisotropy drops sharply below the charge order transition. We interpret our results through a strong electron-phonon scattering picture and find that both electronic and phononic contributions to the diffusivity saturate a proposed bound. Our results suggest that neither well-defined electron nor phonon quasiparticles are present in this material.",1610.05845v2 2016-10-22,High performance THz emitters based on ferromagnetic/nonmagnetic heterostructures,"We report a THz emitter with excellent performances based on nonmagnetic (NM) and ferromagnetic (FM) heterostructures. The spin currents are first excited by the femtosecond laser beam in the NM/FM bilayer, and then transient charge currents are generated by inverse spin Hall effect, leading to THz emission out of the structure. The broadband THz waves emitted from our film stacks have a peak intensity exceeding 500 um thick ZnTe crystals (standard THz emitters). Our device is insensitive to the polarization of an incident laser beam which indicates the noise resistive feature. In contrast, the polarization of THz waves is fully controllable by an external magnetic field. We have also fabricated the devices on flexible substrates with a great performance, and demonstrated that the devices can be driven by low power lasers. Together with the low cost and mass productive sputtering growth method for the film stacks, the proposed THz emitters can be readily applied to a wide range of THz equipment. Our study also points towards an alternative approach to characterize spintronic devices with NM/FM bilayers.",1610.07020v1 2016-10-26,S2DS: Physics-Based Compact Model for Circuit Simulation of Two-Dimensional Semiconductor Devices Including Non-Idealities,"We present a physics-based compact model for two-dimensional (2D) field-effect transistors (FETs) based on monolayer semiconductors such as MoS2. A semi-classical transport approach is appropriate for the 2D channel, enabling simplified analytical expressions for the drain current. In addition to intrinsic FET behavior, the model includes contact resistance, traps and impurities, quantum capacitance, fringing fields, high-field velocity saturation and self-heating, the latter being found to play a strong role. The model is calibrated with state-of-the-art experimental data for n- and p-type 2D-FETs, and it can be used to analyze device properties for sub-100 nm gate lengths. Using the experimental fit, we demonstrate feasibility of circuit simulations using properly scaled devices. The complete model is implemented in SPICE-compatible Verilog-A, and a downloadable version is freely available on the nanoHUB.org.",1610.08489v2 2016-11-14,Nonlinear Transport of Graphene in the Quantum Hall Regime,"We have studied the breakdown of the integer quantum Hall (QH) effect with fully broken symmetry, in an ultra-high mobility graphene device sandwiched between two single crystal hexagonal boron nitride substrates. The evolution and stabilities of the QH states are studied quantitatively through the nonlinear transport with dc Hall voltage bias. The mechanism of the QH breakdown in graphene and the movement of the Fermi energy with the electrical Hall field are discussed. This is the first study in which the stabilities of fully symmetry broken QH states are probed all together. Our results raise the possibility that the v=6 states might be a better target for the quantum resistance standard.",1611.04221v1 2016-11-15,Encapsulated Nanowires: Boosting Electronic Transport in Carbon Nanotubes,"The electrical conductivity of metallic carbon nanotubes (CNTs) quickly saturates with respect to bias voltage due to scattering from a large population of optical phonons. Decay of these dominant scatterers in pristine CNTs is too slow to offset an increased generation rate at high voltage bias. We demonstrate from first principles that encapsulation of 1D atomic chains within a single-walled CNT can enhance decay of ""hot"" phonons by providing additional channels for thermalisation. Pacification of the phonon population growth reduces electrical resistivity of metallic CNTs by 51% for an example system with encapsulated beryllium.",1611.04867v2 2016-12-06,Enhanced Structural Stability and Photo Responsiveness of CH3NH3SnI3 Perovskite via Pressure-Induced Amorphization and Recrystallization,"An organic-inorganic halide perovskite of CH3NH3SnI3 with significantly improved structural stability is obtained via pressure-induced amorphization and recrystallization. In situ high-pressure resistance measurements reveal an increased electrical conductivity by 300% in the pressure-treated perovskite. Photocurrent measurements also reveal a substantial enhancement in visible-light responsiveness. The mechanism underlying the enhanced properties is demonstrated to be associated with the improved structural stability.",1612.01649v1 2016-12-20,Enhanced Superconductivity in TiO Epitaxial Thin Films,"Titanium oxides have many fascinating optical and electrical properties, such as the superconductivity at 2.0 K in cubic titanium monoxide TiO polycrystalline bulk. However, the lack of TiO single crystals or epitaxial films has prevented systematic investigations on its superconductivity. Here, we report the basic superconductivity characterizations of cubic TiO films epitaxially grown on (0001)-oriented Al2O3 substrates. The magnetic and electronic transport measurements confirmed that TiO is a type-II superconductor and the record high Tc is about 7.4 K. The lower critical field (Hc1) at 1.9 K, the extrapolated upper critical field Hc2(0) and coherence length are about 18 Oe, 13.7 T and 4.9 nm, respectively. With increasing pressure, the value of Tc shifts to lower temperature while the normal state resistivity increases. Our results on the superconducting TiO films confirm the strategy to achieve higher Tc in epitaxial films, which may be helpful for finding more superconducting materials in various related systems.",1612.06506v1 2017-02-02,Two-temperature equations of state for d-band metals irradiated by femtosecond laser pulses,"The cold curves for energy and pressure of Copper, Iron, and Tantalum were obtained using methods of the density functional theory. We consider hydrostatic and uniaxial deformations in the range from double compression of the initial volume per atom to double stretching. The presence of allotropic transformation from $\alpha$ - phase of Iron to the hexaferrum with the growth of pressure is observed. In the case of hydrostatic deformations we also have obtained analogous cold curves, but with non-zero electronic temperatures in the range up to 5 eV. The similar volume and electronic temperature ranges have been considered recently. The behavior of electronic internal energy, pressure, and density of states was investigated in the volume and temperature ranges called above. The maximum hydrostatic strains and the types of lattice instabilities were theoretically predicted for the considered metals. The influence of high electronic temperature on the electronic heat conductivity and electric resistivity has been provided for d-band metals by the approach based on the solution of Boltzmann kinetic equation in $\tau$-approximation. This data is compared with the results of quantum molecular dynamics for Gold.",1702.00825v3 2017-02-15,"New bulk p-type skutterudites DD0.7Fe2.7Co1.3Sb12-xXx (X = Ge, Sn) reaching ZT>1.3","The best p-type skutterudites so far are didymium filled, Fe/Co substituted, Sb-based skutterudites. Substitution at the Sb-sites influences the electronic structure, deforms the Sb4-rings, enhances the scattering of phonons on electrons and impurities and this way reduces the lattice thermal conductivity. In this paper we study structural and transport properties of p-type skutterudites with the nominal composition DD0.7Fe2.7Co1.3Sb11.7{Ge/Sn}0.3, which were prepared by a rather fast reaction-annealing-melting technique. The Ge-doped sample showed impurities, which did not anneal out completely and even with ZT > 1 the result was not satisfying. However, the single-phase Sn-doped sample, DD0.7Fe2.7Co1.3Sb11.8Sn0.2, showed a lower thermal and lattice thermal conductivity than the undoped skutterudite leading to a higher ZT=1.3, hitherto the highest ZT for a p-type skutterudite. Annealing at 570 K for 3 days proved the stability of the microstructure. After severe plastic deformation (SPD), due to additionally introduced defects, an enhancement of the electrical resistivity was compensated by a significantly lower thermal conductivity and the net effect led to a record high figure of merit: ZT = 1.45 at 850 K for DD0.7Fe2.7Co1.3Sb11.8Sn0.2.",1702.04498v1 2017-02-24,Out-of-plane easy-axis in thin films of diluted magnetic semiconductor Ba1-xKx(Zn1-yMny)2As2,"Single-phased, single-oriented thin films of Mn-doped ZnAs-based diluted magnetic semiconductor (DMS) Ba1-xKx(Zn1-yMny)2As2 (x = 0.03, 0.08; y = 0.15) have been deposited on Si, SrTiO3, LaAlO3, (La,Sr)(Al,Ta)O3, and MgAl2O4 substrates, respectively. Utilizing a combined synthesis and characterization system excluding the air and further optimizing the deposition parameters, high-quality thin films could be obtained and be measured showing that they can keep inactive-in-air up to more than 90 hours characterized by electrical transport measurements. In comparison with films of x = 0.03 which possess relatively higher resistivity, weaker magnetic performances, and larger energy gap, thin films of x = 0.08 show better electrical and magnetic performances. Strong magnetic anisotropy was found in films of x = 0.08 grown on (La,Sr)(Al,Ta)O3 substrate with their magnetic polarization aligned almost solely on the film growth direction.",1702.07506v1 2017-06-16,An argon ion beam milling process for native $\text{AlO}_\text{x}$ layers enabling coherent superconducting contacts,"We present an argon ion beam milling process to remove the native oxide layer forming on aluminum thin films due to their exposure to atmosphere in between lithographic steps. Our cleaning process is readily integrable with conventional fabrication of Josephson junction quantum circuits. From measurements of the internal quality factors of superconducting microwave resonators with and without contacts, we place an upper bound on the residual resistance of an ion beam milled contact of 50$\,\mathrm{m}\Omega \cdot \mu \mathrm{m}^2$ at a frequency of 4.5 GHz. Resonators for which only $6\%$ of the total foot-print was exposed to the ion beam milling, in areas of low electric and high magnetic field, showed quality factors above $10^6$ in the single photon regime, and no degradation compared to single layer samples. We believe these results will enable the development of increasingly complex superconducting circuits for quantum information processing.",1706.06424v1 2017-06-29,Magnetotransport properties of MoP$_2$,"We report magnetotransport and de Haas-van Alphen (dHvA) effect studies on MoP$_2$ single crystals, predicted to be type-2 Weyl semimetal with four pairs of robust Weyl points located below the Fermi level and long Fermi arcs. The temperature dependence of resistivity shows a peak before saturation, which does not move with magnetic field. Large nonsaturating magnetoresistance (MR) was observed, and the field dependence of MR exhibits a crossover from semicalssical weak-field $B^2$ dependence to the high-field linear-field dependence, indicating the presence of Dirac linear energy dispersion. In addition, systematic violation of Kohler's rule was observed, consistent with multiband electronic transport. Strong spin-orbit coupling (SOC) splitting has an effect on dHvA measurements whereas the angular-dependent dHvA orbit frequencies agree well with the calculated Fermi surface. The cyclotron effective mass $\sim$ 1.6$m_e$ indicates the bands might be trivial, possibly since the Weyl points are located below the Fermi level. Interestingly, quasi-two dimensional(2D) band structure is observed even though the crystal structure of MoP$_2$ is not layered.",1706.09830v1 2017-09-11,Massive fermions with low mobility in antiferromagnet orthorhombic CuMnAs single crystals,"We report the physical properties of orthorhombic o-CuMnAs single crystal, which is predicted to be a topological Dirac semimetal with magnetic ground state and inversion symmetry broken. o-CuMnAs exhibits an antiferromagnetic transition with TN ~ 312 K. Further characterizations of magnetic properties suggest that the AFM order may be canted with the spin orientation in the bc plane. Small isotropic MR and linearly field-dependent Hall resistivity with positive slope indicate that single hole-type carries with high density and low mobility dominate the transport properties of o-CuMnAs. Furthermore, the result of low-temperature heat capacity shows that the effective mass of carriers is much larger than those in typical topological semimetals. These results imply that the carriers in o-CuMnAs exhibit remarkably different features from those of Dirac fermions predicted in theory.",1709.03394v2 2017-09-13,Ultra-broadband photodetectors based on epitaxial graphene quantum dots,"Graphene is an ideal material for hot-electron bolometers, due to its low heat capacity and weak electron-phonon coupling. Nanostructuring graphene with quantum dot constrictions yields detectors with extraordinarily high intrinsic responsivity, higher than 1x10^9 V/W at 3K. The sensing mechanism is bolometric in nature: the quantum confinement gap causes a strong dependence of the electrical resistance on the electron temperature. Here we show that this quantum confinement gap does not impose a limitation on the photon energy for light detection and these quantum dot bolometers work in a very broad spectral range, from terahertz, through telecom to ultraviolet radiation, with responsivity independent of wavelength. We also measure the power dependence of the response. Although the responsivity decreases with increasing power, it stays higher than 1x10^8 V/W in a wide range of absorbed power, from 1 pW to 0.4 nW.",1709.04498v1 2017-09-27,"Pressure-induced Lifshitz transition in NbP: Raman, x-ray diffraction, electrical transport and density functional theory","We report high pressure Raman, synchrotron x-ray diffraction and electrical transport studies on Weyl semimetals NbP and TaP along with first-principles density functional theoretical (DFT) analysis. The frequencies of first-order Raman modes of NbP harden with increasing pressure and exhibit a slope change at P$_c$ $\sim$ 9 GPa, and its resistivity exhibits a minimum at P$_c$. The pressure-dependent volume of NbP exhibits a change in its bulk modulus from 207 GPa to 243 GPa at P$_c$. Using DFT calculations, we show that these anomalies are associated with pressure induced Lifshitz transition which involves appearance of electron and hole pockets in its electronic structure. In contrast, results of Raman and synchrotron x-ray diffraction experiments on TaP and DFT calculations show that TaP is quite robust under pressure and does not undergo any phase transition.",1709.09368v1 2017-10-27,Unusual behavior of cuprates explained by heterogeneous charge localization,"The cuprate high-temperature superconductors are among the most intensively studied materials, yet essential questions regarding their principal phases and the transitions between them remain unanswered. Generally thought of as doped charge-transfer insulators, these complex lamellar oxides exhibit pseudogap, strange-metal, superconducting and Fermi-liquid behaviour with increasing hole-dopant concentration. Here we propose a simple inhomogeneous Mott-like (de)localization model wherein exactly one hole per copper-oxygen unit is gradually delocalized with increasing doping and temperature. The model is percolative in nature, with parameters that are experimentally constrained. It comprehensively captures pivotal unconventional experimental results, including the temperature and doping dependence of the pseudogap phenomenon, the strange-metal linear temperature dependence of the planar resistivity, and the doping dependence of the superfluid density. The success and simplicity of our model greatly demystify the cuprate phase diagram and point to a local superconducting pairing mechanism involving the (de)localized hole.",1710.10221v1 2017-11-05,Investigations of a Robotic Testbed with Viscoelastic Liquid Cooled Actuators,"We design, build, and thoroughly test a new type of actuator dubbed viscoelastic liquid cooled actuator (VLCA) for robotic applications. VLCAs excel in the following five critical axes of performance: energy efficiency, torque density, impact resistence, joint position and force controllability. We first study the design objectives and choices of the VLCA to enhance the performance on the needed criteria. We follow by an investigation on viscoelastic materials in terms of their damping, viscous and hysteresis properties as well as parameters related to the long- term performance. As part of the actuator design, we configure a disturbance observer to provide high-fidelity force control to enable a wide range of impedance control capabilities. We proceed to design a robotic system capable to lift payloads of 32.5 kg, which is three times larger than its own weight. In addition, we experiment with Cartesian trajectory control up to 2 Hz with a vertical range of motion of 32 cm while carrying a payload of 10 kg. Finally, we perform experiments on impedance control and mechanical robustness by studying the response of the robotics testbed to hammering impacts and external force interactions.",1711.01649v2 2017-11-07,Epitaxial stabilization of pulsed laser deposited Sr$_{n+1}$Ir$_n$O$_{3n+1}$ thin films: entangled effect of growth dynamics and strain,"The subtle balance of electronic correlations, crystal field splitting and spin--orbit coupling in layered Ir$^{4+}$ oxides can give rise to novel electronic and magnetic phases. Experimental progress in this field relies on the synthesis of epitaxial films of these oxides. However, the growth of layered iridates with excellent structural quality is a great experimental challenge. Here we selectively grow high quality single--phase films of Sr$_2$IrO$_4$, Sr$_3$Ir$_2$O$_7$, and SrIrO$_3$ on various substrates from a single Sr$_3$Ir$_2$O$_7$ target by tuning background oxygen pressure and epitaxial strain. We demonstrate a complex interplay between growth dynamics and strain during thin film deposition. Such interplay leads to the stabilization of different phases in films grown on different substrates under identical growth conditions, which cannot be explained by a simple kinetic model. We further investigate the thermoelectric properties of the three phases and propose that weak localization is responsible for the low temperature activated resistivity observed in SrIrO$_3$ under compressive strain.",1711.02767v3 2017-11-09,Magnetic phase separation and strong AFM nature of hexagonal Gd$_5$Sb$_3$,"We report on the combined results of structural, magnetic, transport and calorimetric properties of Mn$_5$Si$_3$-type hexagonal Gd$_5$Sb$_3$. With decreasing temperature, it exhibits a ferromagnetic-like transition at 265 K, N\'{e}el transition at 95.5 K and a spin-orientation transition at 62 K. The system is found to be in AFM state down to 2 K in a field of 70 kOe. Magnetic phase coexistence is not noticeable despite large positive Curie-Weiss temperature. Instead low-temperature AFM and high-temperature FM-like phases are separated in large temperature. Temperature-magnetic field ($H$-$T$) phase diagram reveals field-driven complex magnetic phases. Within the AFM phase, the system is observed to undergo field-driven spin-orientation transitions. Field-induced tricritical and quantum critical points appear to be absent due to strong AFM nature and by the intervention of FM-like state between PM and AFM states. Electrical resistivity along with large Sommerfeld parameter suggests metallic nature.",1711.03263v1 2017-11-29,Pressure-induced ferromagnetism due to an anisotropic electronic topological transition in Fe1.08Te,"A rapid and anisotropic modification of the Fermi-surface shape can be associated with abrupt changes in crystalline lattice geometry or in the magnetic state of a material. In this study we show that such an electronic topological transition is at the basis of the formation of an unusual pressure-induced tetragonal ferromagnetic phase in Fe$_{1.08}$Te. Around 2 GPa, the orthorhombic and incommensurate antiferromagnetic ground-state of Fe$_{1.08}$Te is transformed upon increasing pressure into a tetragonal ferromagnetic state via a conventional first-order transition. On the other hand, an isostructural transition takes place from the paramagnetic high-temperature state into the ferromagnetic phase as a rare case of a `type 0' transformation with anisotropic properties. Electronic-structure calculations in combination with electrical resistivity, magnetization, and x-ray diffraction experiments show that the electronic system of Fe$_{1.08}$Te is instable with respect to profound topological transitions that can drive fundamental changes of the lattice anisotropy and the associated magnetic order.",1711.10745v1 2018-01-15,Improving Graphene-metal Contacts: Thermal Induced Polishing,"Graphene is a very promising material for nanoelectronics applications due to its unique and remarkable electronic and thermal properties. However, when deposited on metallic electrodes the overall thermal conductivity is significantly decreased. This phenomenon has been attributed to the mismatch between the interfaces and contact thermal resistance. Experimentally, one way to improve the graphene/metal contact is thorough high-temperature annealing, but the detailed mechanisms behind these processes remain unclear. In order to address these questions, we carried out fully atomistic reactive molecular dynamics simulations using the ReaxFF force field to investigate the interactions between multi-layer graphene and metallic electrodes (nickel) under (thermal) annealing. Our results show that the annealing induces an upward-downward movement of the graphene layers, causing a pile-driver-like effect over the metallic surface. This graphene induced movements cause a planarization (thermal polishing-like effect) of the metallic surface, which results in the increase of the effective graphene/metal contact area. This can also explain the experimentally observed improvements of the thermal and electric conductivities.",1801.04785v1 2018-01-31,Commensurability Oscillations in One-Dimensional Graphene Superlattices,"We report the experimental observation of commensurability oscillations (COs) in 1D graphene superlattices. The widely tunable periodic potential modulation in hBN encapsulated graphene is generated via the interplay of nanopatterned few layer graphene acting as a local bottom gate and a global Si back gate. The longitudinal magneto-resistance shows pronounced COs, when the sample is tuned into the unipolar transport regime. We observe up to six CO minima, providing evidence for a long mean free path despite the potential modulation. Comparison to existing theories shows that small angle scattering is dominant in hBN/graphene/hBN heterostructures. We observe robust COs persisting to temperature exceeding $T=150$ K. At high temperatures, we find deviations from the predicted $T$-dependence, which we ascribe to electron-electron scattering.",1802.00016v2 2018-03-22,High density carriers at a strongly coupled graphene-topological insulator interface,"We report on a strongly coupled bilayer graphene (BLG) - \bise\ device with a junction resistance of less than 1.5 k$\Omega\mu$m$^2$. This device exhibits unique behavior at the interface, which cannot be attributed to either material in absence of the other. We observe quantum oscillations in the magnetoresistance of the junction, indicating the presence of well-resolved Landau levels due to hole carriers of unknown origin with a very large Fermi surface. These carriers, found only at the interface, could conceivably arise due to significant hole doping of the bilayer graphene with charge transfer on the order of 2$\times$10$^{13}$ cm$^{-2}$, or due to twist angle dependent mini-band transport.",1803.08260v1 2018-03-27,Large-Scale Fabrication of RF MOSFETs on Liquid-Exfoliated MoS2,"For the first time, thousands of RF MOSFETs were batch-fabricated on liquid-exfoliated MoS2 below 300 {\deg}C with nearly 100% yield. The large-scale fabrication with high yield allowed the average performance instead of the best performance to be reported. The DC performance of these devices were typical, but the RF performance, enabled by buried gates and on the order of 100 MHz, was reported for the first time for liquid-exfoliated MoS2. To resolve the dilemma of thin vs. thick films, gate recess was used on 20-nm thick films to improve the gate control while keeping the contact resistance lower than that on 10-nm films. These innovations may enable thin-film transistors to operate in the microwave range.",1803.09906v1 2018-05-20,Autonomous actuation of zero modes in mechanical networks far from equilibrium,"A zero mode, or floppy mode, is a non-trivial coupling of mechanical components yielding a degree of freedom with no resistance to deformation. Engineered zero modes have the potential to act as microscopic motors or memory devices, but this requires an internal actuation mechanism that can overcome unwanted fluctuations in other modes and the dissipation inherent in real systems. In this work, we show theoretically and experimentally that complex zero modes in mechanical networks can be selectively mobilized by non-equilibrium activity. We find that a correlated active bath actuates an infinitesimal zero mode while simultaneously suppressing fluctuations in higher modes compared to thermal fluctuations, which we experimentally mimic by high frequency shaking of a physical network. Furthermore, self-propulsive dynamics spontaneously mobilise finite mechanisms as exemplified by a self-propelled topological soliton. Non-equilibrium activity thus enables autonomous actuation of coordinated mechanisms engineered through network topology.",1805.07728v2 2018-06-06,Pressure Evolution of Magnetism in URhGa,"In this paper, we report the results of an ambient and high pressure study of a 5f-electron ferromagnet URhGa. The work is focused on measurements of magnetic and thermodynamic properties of a single crystal sample and on the construction of the p-T phase diagram. Diamond anvil cells were employed to measure the magnetization and electrical resistivity pressures up to ~ 9 GPa. At ambient pressure, URhGa exhibits collinear ferromagnetic ordering of uranium magnetic moments {\mu}U ~ 1.1 {\mu}B (at 2 K) aligned along the c-axis of the hexagonal crystal structure below the Curie temperature TC = 41K. With the application of pressure up to 5GPa the ordering temperature TC initially increases whereas the saturated moment slightly decreases. The rather unexpected evolution is put in the context of the UTX family of compounds.",1806.02686v1 2018-06-25,Ferromagnetism above 1000 K in highly cation-ordered double-perovskite insulator Sr3OsO6,"Magnetic insulators have been intensively studied for over 100 years, and they, in particular ferrites, are considered to be the cradle of magnetic exchange interactions in solids. Their wide range of applications include microwave devices and permanent magnets . They are also suitable for spintronic devices owing to their high resistivity, low magnetic damping, and spin-dependent tunneling probabilities. The Curie temperature is the crucial factor determining the temperature range in which any ferri/ferromagnetic system remains stable. However, the record Curie temperature has stood for over eight decades in insulators and oxides (943 K for spinel ferrite LiFe5O8). Here we show that a highly B-site ordered double-perovskite, Sr2(SrOs)O6 (Sr3OsO6), surpasses this long standing Curie temperature record by more than 100 K. We revealed this B-site ordering by atomic-resolution scanning transmission electron microscopy. The density functional theory (DFT) calculations suggest that the large spin-orbit coupling (SOC) of Os6+ 5d2 orbitals drives the system toward a Jeff = 3/2 ferromagnetic (FM) insulating state. Moreover, the Sr3OsO6 is the first epitaxially grown osmate, which means it is highly compatible with device fabrication processes and thus promising for spintronic applications.",1806.09308v1 2018-06-26,Ultrahigh Magnetic Fields Produced by Shearing Carbon Nanotubes,"In laboratories, ultrahigh magnetic fields are usually produced with very large currents through superconducting, resistive or hybrid magnets, which require extreme conditions, such as low temperature, huge cooling water or tens of megawatts of power. In this work we report that when single walled carbon nanotubes (SWNTs) are cut, there are magnetic moments at the shearing end of SWNTs. The average magnetic moment is found to be 41.5+-9.8uB per carbon atom in the end states with a width of 1 nm at temperature of 300.0K, suggesting ultrahigh magnetic fields can be produced. The dangling sigma and pi bonds of the carbon atoms at the shearing ends play important roles for this unexpectedly high magnetic moments because the oxidation temperature of cut SWNTs is found to be as low as 312 in dry air. Producing ultrahigh magnetic field with SWNTs has the advantage of working at higher working temperature and with low energy consumption, suggesting great potentials of applications.",1806.09891v1 2018-06-27,Slip Detection: Analysis and Calibration of Univariate Tactile Signals,"The existence of tactile afferents sensitive to slip-related mechanical transients in the human hand augments the robustness of grasping through secondary force modulation protocols. Despite this knowledge and the fact that tactile-based slip detection has been researched for decades, robust slip detection is still not an out-of-the-box capability for any commercially available tactile sensor. This research seeks to bridge this gap with a comprehensive study addressing several aspects of slip detection. Key developments include a systematic data collection process yielding millions of sensory data points, the generalized conversion of multivariate-to-univariate sensor output, an insightful spectral analysis of the univariate sensor outputs, and the application of Long Short-Term Memory (LSTM) neural networks on the univariate signals to produce robust slip detectors from three commercially available sensors capable of tactile sensing. The sensing elements underlying these sensors vary in quantity, spatial arrangement, and mechanics, leveraging principles in electro-mechanical resistance, optics, and hydro-acoustics. Critically, slip detection performance of the tactile technologies is quantified through a measurement methodology that unveils the effects of data window size, sampling rate, material type, slip speed, and sensor manufacturing variability. Results indicate that the investigated commercial tactile sensors are inherently capable of high-quality slip detection.",1806.10451v1 2018-06-27,Electron-hole tunneling revealed by quantum oscillations in the nodal-line semimetal HfSiS,"We report a study of quantum oscillations in the high-field magneto-resistance of the nodal-line semimetal HfSiS. In the presence of a magnetic field up to 31 T parallel to the c-axis, we observe quantum oscillations originating both from orbits of individual electron and hole pockets, and from magnetic breakdown between these pockets. In particular, we find an oscillation associated with a breakdown orbit enclosing one electron and one hole pocket in the form of a `figure of eight'. This observation represents an experimental confirmation of the momentum space analog of Klein tunneling. When the c-axis and the magnetic field are misaligned with respect to one another, this oscillation rapidly decreases in intensity. Finally, we extract the cyclotron masses from the temperature dependence of the oscillations, and find that the mass of the 'figure of eight' orbit corresponds to the sum of the individual pockets, consistent with theoretical predictions for Klein tunneling in topological semimetals.",1806.10592v1 2018-06-28,Bloch surface waves at the telecommunication wavelength with Lithium Niobate as top layer for integrated optics,"Lithium niobate (LN) based devices are widely used in integrated and nonlinear optics. This material is robust and resistive to high temperatures, which makes the LN-based devices table, but challenging to fabricate. In this work we report on the design, manufacturing and characterization of engineered dielectric media with thin film lithium niobate (TFLN) on top for the coupling and propagation of electromagnetic surface waves at the telecommunication wavelengths. The designed one-dimentional photonic crystal (1DPhC) sustains Bloch surface waves at the multilayer/air interface at 1550 nm wavelength with a propagation detected over a distance of 3 mm. The working wavelength and improved BSW propagation parameters open the way for exploration of nonlinear properties of BSW based devices. It is also expected that these novel devices will modify BSW propagation and coupling by external thermal/electrical stimuli due to the improved quality of the TFLN top layer of 1DPhC.",1806.11142v1 2018-11-06,Low-dispersion low-loss dielectric gratings for efficient ultrafast laser pulse compression at high average powers,"We have developed low-dispersion (1480 l/mm), resonance-free, diffraction gratings made of dielectric materials resistant to femtosecond laser damage $(SiO_{2}/HfO_{2})$. A 14 cm diameter sample was fabricated resulting in a mean diffraction efficiency of 99.1% at {\lambda} = 810 nm with 0.4% uniformity using equipment which can fabricate gratings up to 1m diagonal. The implementation of these gratings in the compression of 30 fs pulses in an out-of-plane geometry can result in compressor efficiencies of ~95%. The measured laser absorption is 500x lower than current ultrafast petawatt-class compressor gratings which will enable a substantial increase in average power handling capabilities of these laser systems.",1811.03091v1 2018-11-13,Fermi- to non-Fermi-liquid crossover and Kondo transition in two-dimensional Cu$_{2/3}$V$_{1/3}$V$_2$S$_4$,"By means of a specific heat ($C$) and electrical resistivity ($\varrho$) study, we give evidence of a pronounced Fermi liquid (FL) behavior with sizable mass renormalization, $m^{\ast}/m = 30$, up to unusually high temperatures $\sim$70 K in the layered system Cu$_{2/3}$V$_{1/3}$V$_2$S$_4$. At low temperature, a marked upturn of both $C$ and $\varrho$ is suppressed by magnetic field, which suggests a picture of Kondo coupling between conduction electrons in the VS$_2$ layers and impurity spins of the V$^{3+}$ ions located between layers. This picture opens the possibility of controlling electronic correlations and the FL to non-FL crossover in simple layered materials. For instance, we envisage that the coupling between layers provided by the impurity spins may realize a two-channel Kondo state.",1811.05431v1 2019-05-09,A lower bound to the thermal diffusivity of insulators,"It has been known for decades that thermal conductivity of insulating crystals becomes proportional to the inverse of temperature when the latter is comparable to or higher than the Debye temperature. This behavior has been understood as resulting from Umklapp scattering among phonons. We put under scrutiny the magnitude of the thermal diffusion constant in this regime and find that it does not fall below a threshold set by the square of sound velocity times the Planckian time ($\tau_p=\hbar/k_BT$). The conclusion, based on scrutinizing the ratio in cubic crystals with high thermal resistivity, appears to hold even in glasses where Umklapp events are not conceivable. Explaining this boundary, reminiscent of a recently-noticed limit for charge transport in metals, is a challenge to theory.",1905.03551v3 2019-05-19,Unraveling the Effect of Electron-Electron Interaction on Electronic Transport in High-Mobility Stannate Films,"Contrary to the common belief that electron-electron interaction (EEI) should be negligible in s-orbital-based conductors, we demonstrated that the EEI effect could play a significant role on electronic transport leading to the misinterpretation of the Hall data. We show that the EEI effect is primarily responsible for an increase in the Hall coefficient in the La-doped SrSnO3 films below 50 K accompanied by an increase in the sheet resistance. The quantitative analysis of the magnetoresistance (MR) data yielded a large phase coherence length of electrons exceeding 450 nm at 1.8 K and revealed the electron-electron interaction being accountable for breaking of electron phase coherency in La-doped SrSnO3 films. These results while providing critical insights into the fundamental transport behavior in doped stannates also indicate the potential applications of stannates in quantum coherent electronic devices owing to their large phase coherence length.",1905.07810v1 2019-05-30,Molecular Beam Epitaxy Growth of Antiferromagnetic Kagome Metal FeSn,"FeSn is a room-temperature antiferromagnet expected to host Dirac fermions in its electronic structure. The interplay of magnetic degree of freedom and the Dirac fermions makes FeSn an attractive platform for spintronics and electronic devices. While stabilization of thin film FeSn is needed for the development of such devices, there exist no previous report of epitaxial growth of single crystalline FeSn. Here we report the realization of epitaxial thin films of FeSn (001) grown by molecular beam epitaxy on single crystal SrTiO$_{3}$ (111) substrates. By combining X-ray diffraction, electrical transport, and torque magnetometry measurements, we demonstrate the high quality of these films with the residual resistivity ratio $\rho_{xx}(300 \hspace{0.2em}{\rm K})/\rho_{xx}(2 \hspace{0.2em}{\rm K}) = 24$ and antiferromagnetic ordering at $T_{\rm N}$ = 353 K. These developments open a pathway to manipulate the Dirac fermions in FeSn by both magnetic interactions and the electronic field effect for use in antiferromagnetic spintronics devices.",1905.13073v1 2019-09-20,Pressure-tunable large anomalous Hall effect of the ferromagnetic kagome-lattice Weyl semimetal Co3Sn2S2,"We investigate the pressure evolution of the anomalous Hall effect in magnetic topological semimetal Co3Sn2S2 in diamond anvil cells with pressures up to 44.9-50.9 GPa. No evident trace of structural phase transition is detected through synchrotron x-ray diffraction over the measured pressure range of 0.2-50.9 GPa. We find that the anomalous Hall resistivity and the ferromagnetism are monotonically suppressed as increasing pressure and almost vanish around 22 GPa. The anomalous Hall conductivity varies non-monotonically against pressure at low temperatures, involving competition between original and emergent Weyl nodes. Combined with first-principle calculations, we reveal that the intrinsic mechanism due to the Berry curvature dominates the anomalous Hall effect under high pressure.",1909.09382v1 2019-09-22,Robust pseudogap across the magnetic field driven superconductor to insulator-like transition in strongly disordered NbN films,"We investigate the magnetic field evolution of the superconducting state in a strongly disordered NbN thin film which exhibits a magnetic field tuned superconductor to insulator-like transition, employing low temperature scanning tunneling spectroscopy (STS). Transport measurements of the sample reveals a characteristic magnetic field, which separates the low field state where resistance decreases with decreasing temperature, i.e. dR/dT > 0 and a high-field state where dR/dT < 0. However, STS imaging of the superconducting state reveals a smooth evolution across this field and the presence of a robust pseudogap on both sides of this characteristic field. Our results suggest that the superconductor-insulator transition might be a percolative transition driven by the shrinking of superconducting fraction with magnetic field.",1909.10071v1 2020-03-04,High-Performance Atomically-Thin Room-Temperature NO2 Sensor,"The development of room-temperature sensing devices for detecting small concentrations of molecular species is imperative for a wide range of low-power sensor applications. We demonstrate a room-temperature, highly sensitive, selective, and reversible chemical sensor based on a monolayer of the transition metal dichalcogenide Re0.5Nb0.5S2. The sensing device exhibits thickness dependent carrier type, and upon exposure to NO2 molecules, its electrical resistance considerably increases or decreases depending on the layer number. The sensor is selective to NO2 with only minimal response to other gases such as NH3, CH2O, and CO2. In the presence of humidity, not only are the sensing properties not deteriorated, but also the monolayer sensor shows complete reversibility with fast recovery at room temperature. We present a theoretical analysis of the sensing platform and identify the atomically-sensitive transduction mechanism.",2003.01909v2 2020-03-17,Measurement of the heat flux normalised spin Seebeck coefficient of thin films as a function of temperature,"The spin Seebeck effect (SSE) has generated interest in the thermoelectric and magnetic communities for potential high efficiency energy harvesting applications, and spintronic communities as a source of pure spin current. To understand the underlying mechanisms requires characterisation of potential materials across a range of temperatures, however, for thin films the default measurement of an applied temperature gradient (across the sample) has been shown to be compromised by the presence of thermal resistances. Here, we demonstrate a method to perform low temperature SSE measurements where instead of monitoring the temperature gradient, the heat flux passing through the sample is measured using two calibrated heat flux sensors. This has the advantage of measuring the heat loss through the sample as well as providing a reliable method to normalise the SSE response of thin film samples. We demonstrate this method with an $\text{SiO}_{2}/\text{Fe}_{3}O_{4}/\text{Pt}$ sample, where a semiconducting-insulating transition occurs at the Verwey transition, $T_{\text{V}}$, of $\text{Fe}_{3}\text{O}_{4}$ and quantify the thermomagnetic response above and below $T_{\text{V}}$.",2003.07925v1 2020-03-25,Dualism of the 4f electrons and high-temperature antiferromagnetism of the heavy-fermion compound YbCoC$_{2}$,"We report on the first study of the noncentrosymmetric ternary carbide YbCoC$_{2}$. Our magnetization, specific heat, resistivity and neutron diffraction measurements consistently show that the system behaves as a heavy-fermion compound, displaying an amplitude-modulated magnetic structure below the N\'eel temperature reaching $T_{N}$ = 33 K under pressure. Such a large value, being the highest among the Yb-based systems, is explained in the light of our ab initio calculations, which show that the 4f electronic states of Yb have a dual nature -- i.e., due to their strong hybridization with the 3d states of Co, 4f states expose both localized and itinerant properties.",2003.11601v1 2014-08-13,Crossover from charge order to strain glass in phase separated manganite thin films: Impact of thermal cycling and substrate induced strain,"The magnetic and magnetotransport properties of single crystalline La1-x-yPryCaxMnO3 (x=0.42, y=0.40) thin films (~140 nm) deposited on (110) oriented LaAlO3 and SrTiO3 substrates exhibit a crossover from the high temperature antiferromagnetic-charge ordered insulator (AFM-COI) phase (T>TN) to strain glass (T 95% assuming identical interfaces. These results show that uniaxial anisotropy is not necessary for large TMR, and lay the groundwork for future improvements in TMR in manganite junctions.",1104.1072v1 2011-04-07,Electrostatic Control of the Evolution from Superconductor to Insulator in Ultrathin Films of Yttrium Barium Copper Oxide,"The electrical transport properties of ultrathin YBCO films have been modified using an electric double layer transistor configuration employing an ionic liquid. The films were grown on SrTiO3 substrates using high pressure oxygen sputtering. A clear evolution from superconductor to insulator was observed in nominally 7 unit cell thick films. Using a finite size scaling analysis, curves of resistance versus temperature, R(T), over the temperature range from 6K to 22K were found to collapse onto a single scaling function, which suggests the the presence of a quantum critical point. However the scaling failed at the lowest temperatures suggesting the presence of an additional phase between the superconducting and insulating regimes.",1104.1357v1 2011-04-07,Interference effects in phtalocyanine controlled by H-H tautomerization: a potential two-terminal unimolecular electronic switch,"We investigate the electrical transport properties of two hydrogen tautomer configurations of phthalocyanine (H2Pc) connected to cumulene and gold leads. Hydrogen tautomerization affects the electronic state of H2Pc by switching the character of molecular orbitals with the same symmetry close to the Fermi level. The near degeneracy between the HOMO and HOMO-1 leads to pronounced interference effects, causing a large change in current for the two tautomer configuratons, especially in the low-bias regime. Two types of planar junctions are considered: cumulene-H2Pc-cumulene and gold-H2Pc-gold. Both demonstrate prominent difference in molecular conductance between ON and OFF states. In addition, junctions with gold leads show pronounced negative differential resistance (NDR) at high bias voltage, as well as weak NDR at intermediate bias.",1104.1441v2 2012-03-07,Hall helps Ohm: some corrections to negative-U centers approach to transport properties of YBa$_2$Cu$_3$O$_x$ and La$_{2-x}$Sr$_x$CuO$_4$,"For broad oxygen and strontium doping ranges, temperature dependences (T-dependences) of the normal state resistivity \rho(T) of YBa_2Cu_3O_x (YBCO) and La_(2-x)Sr_xCuO_4 (LSCO) are calculated and compared to experiments. Holes transport was taken in the \tau-approximation, where \tau(T,\epsilon) is due to acoustic phonons. Besides, T-dependence of the chemical potential \mu(T) and effective carrier mass m* ~10-100 free electron masses, obtained by negative-U centers modelling the T-dependence of the Hall coefficient, were used to calculate \rho(T). In addition, it is demonstrated that anisotropy of the cuprates does not affect the calculated T-variation of neither Hall coefficient nor \rho, but only rescale their magnitudes by factors depending on combinations of m_ab and m_c.",1203.1579v1 2012-03-29,Fermi level tuning and a large activation gap achieved in the topological insulator Bi_{2}Te_{2}Se by Sn doping,"We report the effect of Sn doping on the transport properties of the topological insulator Bi_{2}Te_{2}Se studied in a series of Bi_{2-x}Sn_{x}Te_{2}Se crystals with 0 \leq x \leq 0.02. The undoped stoichiometric compound (x = 0) shows an n-type metallic behavior with its Fermi level pinned to the conduction band. In the doped compound, it is found that Sn acts as an acceptor and leads to a downshift of the Fermi level. For x \geq 0.004, the Fermi level is lowered into the bulk forbidden gap and the crystals present a resistivity considerably larger than 1 Ohmcm at low temperatures. In those crystals, the high-temperature transport properties are essentially governed by thermally-activated carriers whose activation energy is 95-125 meV, which probably signifies the formation of a Sn-related impurity band. In addition, the surface conductance directly obtained from the Shubnikov-de Haas oscillations indicates that a surface-dominated transport can be achieved in samples with several um thickness.",1203.6411v1 2015-04-14,Pressure Induced Enhancement of Superconductivity in LaRu2P2,"To explore new superconductors beyond the copper-based and iron-based systems is very important. The Ru element locates just below the Fe in the periodic table and behaves like the Fe in many ways. One of the common thread to induce high temperature superconductivity is to introduce moderate correlation into the system. In this paper, we report the significant enhancement of superconducting transition temperature from 3.84K to 5.77K by using a pressure only of 1.74 GPa in LaRu2P2 which has an iso-structure of the iron-based 122 superconductors. The ab-initio calculation shows that the superconductivity in LaRu2P2 at ambient pressure can be explained by the McMillan's theory with strong electron-phonon coupling. However, it is difficult to interpret the significant enhancement of Tc versus pressure within this picture. Detailed analysis of the pressure induced evolution of resistivity and upper critical field Hc2(T) reveals that the increases of Tc with pressure may be accompanied by the involvement of extra electronic correlation effect. This suggests that the Ru-based system has some commonality as the Fe-based superconductors.",1504.03652v1 2015-04-16,Electron mobility in InxGa1-xN channel HEMTs,"In this letter, we report on the theoretical investigations of electron mobility in practically viable designs of InxGa1-xN channel high electron mobility transistors (HEMT). Carriers in such devices are expected to exhibit a higher velocity and hence higher cut-off frequencies (fT) for highly scaled architectures. We estimate that the mobility of two dimensional electron gas (2DEG) is limited by alloy scattering rather than phonon scattering unlike in conventional GaN-channel HEMTs. For indium composition of 0.30, the mobility and sheet resistance are found to be 500 cm2/Vs and 700 ohm per sq. respectively, which can severely affect the parasitic voltage drop in access regions. The results presented here are believed to significantly guide the practical exploration of InxGa1-xN channel HEMTs towards next-generation electronics by enabling careful design of device layouts in highly scaled transistors to minimize parasitic access region voltage drop which results due to significant degradation of 2DEG mobility.",1504.04336v1 2015-06-01,Topological stability versus thermal agitation in a metastable magnetic skyrmion lattice,"Topologically stable matters can have a long lifetime, even if thermodynamically costly, when the thermal agitation is sufficiently low. A magnetic skyrmion lattice (SkL) represents a unique form of long-range magnetic order that is topologically stable, and therefore, a long-lived, metastable SkL can form. Experimental observations of the SkL in bulk crystals, however, have mostly been limited to a finite and narrow temperature region in which the SkL is thermodynamically stable; thus, the benefits of the topological stability remain unclear. Here, we report a metastable SkL created by quenching a thermodynamically stable SkL. Hall-resistivity measurements of MnSi reveal that, although the metastable SkL is short-lived at high temperatures, the lifetime becomes prolonged (>> 1 week) at low temperatures. The manipulation of a delicate balance between thermal agitation and the topological stability enables a deterministic creation/annihilation of the metastable SkL by exploiting electric heating and subsequent rapid cooling, thus establishing a facile method to control the formation of a SkL.",1506.00363v2 2015-07-02,Wavelength tuning and stabilization of microring-based filters using silicon in-resonator photoconductive heaters,"We demonstrate that n-doped resistive heaters in silicon waveguides show photoconductive effects with high responsivities. These photoconductive heaters, integrated into microring resonator (MRR)-based filters, were used to automatically tune and stabilize the filter's resonance wavelength to the input laser's wavelength. This is achieved without requiring dedicated defect implantations, additional material depositions, dedicated photodetectors, or optical power tap-outs. Automatic wavelength stabilization of first-order MRR and second-order series-coupled MRR filters is experimentally demonstrated. Open eye diagrams were obtained for data transmission at 12.5 Gb/s while the temperature was varied by 5 C at a rate of 0.28 C/s. We theoretically show that series-coupled MRR-based filters of any order can be automatically tuned by using photoconductive heaters to monitor the light intensity in each MRR, and sequentially aligning the resonance of each MRR to the laser's wavelength.",1507.00686v2 2015-07-18,Addressing the Challenges of Using Ferromagnetic Electrodes in the Molecular Spintronics Devices,"Ferromagnetic electrodes chemically bonded with thiol functionalized molecules can produce novel molecular spintronics devices. However, major challenges lie in developing Ferromagnetic electrodes based commercially viable device fabrication scheme that consider the susceptibility of ferromagnetic electrodes to oxidation, chemical etching, and stress induced deformations during fabrication and usage. This paper studies NiFe, an alloy used in the present day memory devices and high-temperature engineering applications, as a candidate FM electrode for the fabrication of MSDs. Our spectroscopic reflectance studies show that NiFe start oxidizing aggressively beyond 90 C. The NiFe surfaces, aged for several months or heated for several minutes below 90 C, exhibited remarkable electrochemical activity and were suitable for chemical bonding with the thiol functionalized molecular device elements. NiFe also demonstrated excellent etching resistance and minimized the mechanical stress induced deformities. This paper demonstrates the successful utilization of NiFe electrodes in the tunnel junction based molecular device fabrication approach. This paper is expected to fill the knowledge gap impeding the experimental development of ferromagnetic electrode based molecular spintronics devices for realizing novel logic and memory devices and observing a numerous theoretically predicted phenomenon.",1507.05146v1 2015-07-26,Topological Phase Transition in Single Crystals of $(Cd_{1-x} Zn_x)_3 As_2$,"Single crystals of $(Cd_{1-x} Zn_x)_3 As_2$ were synthesized from high-temperature solutions and characterized in terms of their structural and electrical properties. Based on the measurements of resistivity and Hall signals, we revealed a chemical-doping-controlled transition from a three dimensional Dirac semimetal to a semiconductor with a critical point $x_c/sim 0.38$. We observed structural transitions from a body-center tetragonal phase to a primary tetragonal phase then back to a body-center tetragonal phase in the solid solutions as well, which are irrelevant to the topological phase transition. This continuously tunable system controlled by chemical doping provides a platform for investigating the topological quantum phase transition of 3D Dirac electrons.",1507.07169v1 2016-09-08,Collective Dynamics and Strong Pinning near the Onset of Charge Order in La$_{1.48}$Nd$_{0.4}$Sr$_{0.12}$CuO$_{4}$,"The dynamics of charge-ordered states is one of the key issues in underdoped cuprate high-temperature superconductors, but static short-range charge-order (CO) domains have been detected in almost all cuprates. We probe the dynamics across the CO (and structural) transition in La$_{1.48}$Nd$_{0.4}$Sr$_{0.12}$CuO$_{4}$ by measuring nonequilibrium charge transport, or resistance $R$ as the system responds to a change in temperature and to an applied magnetic field. We find evidence for metastable states, collective behavior, and criticality. The collective dynamics in the critical regime indicates strong pinning by disorder. Surprisingly, nonequilibrium effects, such as avalanches in $R$, are revealed only when the critical region is approached from the charge-ordered phase. Our results on La$_{1.48}$Nd$_{0.4}$Sr$_{0.12}$CuO$_{4}$ provide the long-sought evidence for the fluctuating order across the CO transition, and also set important constraints on theories of dynamic stripes.",1609.02591v3 2016-09-21,Change-over of carrier type and magneto-transport property in Cu doped Bi2Te3 Topological Insulators,"Structural, resistivity, thermoelectric power and magneto-transport properties of Cu doped Bi2Te3 topological insulators have been investigated. The occurrence of the tuning of charge carriers from n type to p type by Cu doping at Te sites of Bi2Te3 is observed both from Hall effect and thermoelectric power measurements. Carrier mobility decreases with the doping of Cu which provides evidence of the movement of Fermi level from bulk conduction band to the bulk valence band. Thermoelectric power also increaseswith doping of Cu.Moreover linear magnetoresistance (LMR) has been observed at high magnetic field in pure Bi2Te3 which is associated to the gapless topological surface states protected by time reversal symmetry (TRS), whereas doping of Cu breaks TRS and an opening of band gap occurs which quenches the LMR.",1609.06542v1 2016-09-26,Anisotropic heat conduction in silicon nanowire network revealed by Raman scattering,"Anisotropic nanomaterials possess interesting thermal transport properties because they allow orientation of heat fluxes along preferential directions due to a high ratio (up to three orders of magnitude) between their in-plane and cross-plane thermal conductivities. Among different techniques allowing thermal conductivity evaluation, micro-Raman scattering is known to be one of the most efficient contactless measurement approaches. In this letter, a new experimental approach based on Raman scattering measurements with variable laser spot sizes is reported. Correlation between experimental and calculated thermal resistances of one-dimensional nanocrystalline solids allows simultaneous estimation of their in-plane and cross-plane thermal conductivities. In particular, our measurement approach is illustrated to be successfully applied for anisotropic thermal conductivity evaluation of silicon nanowire arrays.",1609.08133v3 2016-09-27,Lifshitz Transitions in the Ferromagnetic Superconductor UCoGe,"We present high field magnetoresistance, Hall effect and thermopower measurements in the Ising-type ferromagnetic superconductor UCoGe. Magnetic field is applied along the easy magnetization $c$ axis of the orthorhombic crystal. In the different experimental probes we observed five successive anomalies at $H \approx 4$, 9, 12, 16, and 21~T. Magnetic quantum oscillations were detected both in resistivity and thermoelectric power. At most of the anomalies, significant changes of the oscillation frequencies and the effective masses have been observed indicating successive Fermi surface instabilities induced by the strong magnetic polarization under magnetic field.",1609.08466v1 2018-07-07,Oxygen Potential Transition in Mixed Conducting Oxide Electrolyte,"It is generally assumed that oxygen potential in a thin oxide electrolyte follows a linear distribution between electrodes. Jacobsen and Mogensen have shown, however, that this is not the case for thin zirconia membranes in solid oxide electrochemical cells. Here we demonstrate that there is a ubiquitous oxygen potential transition rooted in the p-type/n-type transition of electronic conductivity inside mixed conducting oxides, and that the transition is extremely sensitive to electrode potential and current density. It is also remarkably sensitive to the conductivity ratio of electrons and holes, as well as their association with lattice oxygens and vacancies, which tends to increase the oxygen flow. Direct evidence of a sharp oxygen potential transition has been found in an equally sharp grain size transition in electrically loaded zirconia. More broadly speaking, the oxygen potential transition is akin to a first-order phase transition. Therefore, it will suffer interface instability, especially in high-current-density devices. These findings provide new opportunities to understand several disparate observations in the literature, from microstructural degradation and stress distribution in solid oxide fuel/electrolyzer cells, to field-assisted sintering, to conducting filaments in resistance memory, to dendrite formation in electrochemical cells.",1807.02704v1 2018-07-31,Visible absorbing TiO2 thin films by physical deposition methods,"Titanium dioxide is one of the most widely used wide bandgap materials. However, the TiO2 deposited on a substrate is not always transparent leading to a loss in efficiency of the device, especially, the photo response. Herein, we show that atomic layer deposition (ALD) and sputtered TiO2 thin films can be highly absorbing in the visible region. While in ALD, the mechanism is purported to be due to oxygen deficiency, intriguingly, in sputtered films it has been observed that in fact oxygen rich atmosphere leads to visible absorption. We show that the oxygen content during deposition, the resistivity of the film could be controlled and also the photocatalysis response has been evaluated for both the ALD and sputtered films. High resolution TEM and STEM studies show that the origin of visible absorption could be due to the presence of nanoparticles with surface defects inside the amorphous film.",1807.11748v1 2018-12-03,Anomalous scalings of the cuprate strange metals from nonlinear electrodynamics,"We examine transport in a holographic model which describes, through a nonlinear gauge field sector, generic nonlinear interactions between the charge carriers. Scaling exponents are introduced by using geometries which are nonrelativistic and hyperscaling-violating in the infrared. In the dilute charge limit in which the gauge field sector does not backreact on the geometry, a particularly simple nonlinear theory reproduces the anomalous temperature dependence of the resistivity and Hall angle of the cuprate strange metals, $R \sim T$ and $\cot\Theta_H \sim T^2$ while also allowing for a linear entropy $S \sim T$, and predicts that the magnetoresistance for small values of the magnetic field $h$ should scale as $\sim h^2 T^{-4}$. Our study lends evidence to the idea that the strange metal behavior of the cuprates relies crucially on the linear temperature dependence of the entropy.",1812.01040v2 2018-12-17,PNADIS: An automated Peierls-Nabarro Analyzer for DISlocation core structure and slip resistance,"Dislocation is one of the most critical and fundamental crystal defects that dominate the mechanical behavior of crystalline solids, however, a quantitative determination of its character and property in experiments is quite challenging and limited so far. In this paper, a fully automated Peierls-Nabarro (P-N) analyzer named PNADIS is presented; a complete set of the character and property of dislocation can be automatically derived, including the dislocation core structure, Peierls energy and stress, pressure field around dislocation core, solute/dislocation interaction energy, as well as the energy barrier and yield stress at 0K for solid solution strengthening. Furthermore, both one-dimensional (1D) and two-dimensional (2D) P-N models are implemented to meet the demand to analyze the character and property of dislocation for not only simple FCC and HCP structures but also complex crystals. The implementation of this code has been critically validated by a lot of evaluations and tests including 1D P-N model for complex crystals, 2D P-N model for FCC and HCP metals, pressure field around dislocation core, and solid solution strengthening for alloys. We expect that the automated feature of this code would provide a high-efficiency solution for determining the character and property of dislocation.",1812.06630v1 2019-01-23,Stacking of nanocrystalline graphene for Nano-Electro-Mechanical (NEM) actuator applications,"Graphene nano-electro-mechanical switches are promising components due to their excellent switching performance such as low pull-in voltage and low contact resistance. Mass fabrication with an appropriate counter electrode remains challenging. In this work, we report the stacking of nanocrystalline graphene (NCG) with a 70-nm dielectric separation layer. The buried NCG layer is contacted through the formation of vias and acts as actuation electrode. After metallization, the top 7.5-nm thin NCG layer is patterned to form double-clamped beams, and the structure is released by hydrofluoric acid etching. By applying a voltage between the top and buried NCG layer, a step-like current increase is observed below 1.5 V, caused by the contact of the movable beam with the buried NCG. No pull-out is observed due to the thin sacrificial layer and high beam length, resulting in low mechanical restoring force. We discuss the possible applications of the NCG stacking approach to realize Nano-Electro-Mechanical (NEM) contact switches and advanced logical components such as a AND logic.",1901.07754v1 2019-06-10,Successive Symmetry Breaking in a Jeff = 3/2 Quartet in the Spin-Orbit Coupled Insulator Ba2MgReO6,"We report on the cubic double perovskite Ba2MgReO6 containing Re6+ ions with the 5d1 electron configuration. Resistivity, magnetization, and heat capacity measurements using single crystals show that the compound is a Mott insulator with a magnetic transition at Tm = 18 K, which is accompanied by a weak ferromagnetic moment with [110] anisotropy. Another transition is observed at Tq = 33 K in heat capacity, where the inverse of magnetic susceptibility changes its slope, indicating a substantial change in the electronic state. The significance of spin-orbit coupling is revealed by the reduced effective magnetic moment of ~0.68{\mu}B at high temperature above Tq and the total electronic entropy close to Rln4. These features indicate that Ba2MgReO6 is a spin-orbit coupled Mott insulator possessing a Jeff = 3/2 quartet state, which exhibits quadrupolar and dipolar orders at Tq and Tm, respectively.",1906.03802v1 2019-10-07,Ultrasound homogenises suspensions of hydrophobic particles,"Hydrophobic particles inherently resist being suspended. Hydrophobic particles might be regarded as tiny solid particles surrounded by a thin gaseous shell. It has been hypothesised that hydrophobic particles act as cavitation nuclei. This cavitation behaviour would explain the translation speeds observed when hydrophobic polystyrene microspheres were driven through a liquid medium by means of ultrasound. These translation speeds corresponded to those observed with gas microbubbles of similar sizes. If hydrophobic particles do have a thin gaseous layer surrounding the solid cores, a sound field of sufficient pressure amplitude might force the gas layer to form and inertial cavity and subsequently fragment during the collapse phase. In this study, we investigated whether hydrophobic particles can be forced to suspend by using ultrasound. Hydrophobic particles of the materials C65 and ZnO can be forced to be suspended in water using ultrasound. The high-speed observations confirm that hydrophobic particles can act as cavitation nuclei. The lack of cavitation after the first pulse indicates that the gas layer surrounding the hydrophobic particle dissolves after inertial cavitation.",1910.02714v2 2019-10-19,Wafer-size VO2 film prepared by water-vapor oxidant,"The growth of wafer-scale and uniform monoclinic VO2 film was a challenge if considering the multivalent vanadium atom and the various phase structures of VO2 compound. Directly oxidizing metallic vanadium film in oxygen gas seemed to be an easy way, while the oxidation parameters were extremely sensitive due to the critical preparation window. Here we proposed a facile thermal oxidation by water-vapor to produce wafer-scale VO2 films with high quality. Results indicated that by using the water-vapor oxidant, the temperature window for VO2 growth was greatly broadened. In addition, the obtained wafer-size VO2 film showed very uniform surface and sharp resistance change. The chemical reaction routes with water-vapor were calculated, which favored the VO2 film growth. Our results not only demonstrated that the water-vapor could be used as a modest oxidizing agent, but also showed the unique advantage for large size VO2 film preparation.",1910.08776v3 2019-10-28,Hikami-Larkin-Nagaoka (HLN) Fitting of Magneto Transport of Bi2Se3 Single Crystal in Different Magnetic Field Ranges,"We report the detailed study of structural micro-structuraland high magnetic field magneto transport propertiesof Bi2Se3single crystal. Bi2Se3 single crystal is grown through conventional solid-state reaction route via the self-flux method. Rietveld analysis on Powder X-ray Diffraction showed that the studied Bi2Se3 crystal is crystallized in single-phase without any impurity. The surface morphology analyzed through Scanning Electron Microscopy study which shows that as-grown single crystal exhibit layered type structure and the quantitative weight of the atomic constituents (Bi and Se) are found to be closeto the stoichiometric amount in energy-dispersive X-ray spectroscopy analysis. Low temperature (2.5K) magneto-resistance (MR) exhibited a v-type cusp around origin at lower magnetic field, which is the sign of weak anti-localization effect. Further, Bi2Se3 single crystal magneto conductivity data is fitted by well-known HLN equation in different magnetic field range of 2Tesla, 4Tesla and 6Tesla and the resultant found that the conduction mechanism of Bi2Se3 is dominated by WAL state.",1910.12438v1 2019-11-06,Microscopic charging and in-gap states in superconducting granular aluminum,"Following the emergence of superconducting granular aluminum (grAl) as a material for high-impedance quantum circuits, future development hinges on a microscopic understanding of its phase diagram, and whether the superconductor-to-insulator transition (SIT) is driven by disorder or charging effects. Beyond fundamental relevance, these mechanisms govern noise and dissipation in microwave circuits. Although the enhancement of the critical temperature, and the SIT in granular superconductors have been studied for more than fifty years, experimental studies have so far provided incomplete information on the microscopic phenomena. Here we present scanning tunneling microscope measurements of the local electronic structure of superconducting grAl. We confirm an increased superconducting gap in individual grains both near and above the Mott resistivity $\rho_\mathrm{M} \approx 400\ \mu \Omega cm$. Above $\rho_\mathrm{M}$ we find Coulomb charging effects, a first indication for decoupling, and in-gap states on individual grains, which could contribute to flux noise and dielectric loss in quantum devices. We also observe multiple low-energy states outside the gap, which may indicate bosonic excitations of the superconducting order parameter.",1911.02312v2 2019-11-14,GFET Asymmetric Transfer Response Analysis through Access Region Resistances,"Graphene-based devices are planned to augment the functionality of Si and III-V based technology in radio-frequency (RF) electronics. The expectations in designing graphene {field-effect} transistors (GFETs) with enhanced RF performance have attracted significant experimental efforts, mainly concentrated on achieving high mobility samples. However, little attention has been paid, so far, to the role of the access regions in these devices. \mbox{Here, we analyse} in detail, via numerical simulations, how the GFET transfer response is severely impacted by these regions, showing that they play a significant role in the asymmetric saturated behaviour commonly observed in GFETs. We also investigate how the modulation of the access region conductivity (i.e., by the influence of a back gate) and the presence of imperfections in the graphene layer (e.g., charge puddles) affects the transfer response. The analysis is extended to assess the application of GFETs for RF applications, by~evaluating their cut-off frequency.",1911.06360v1 2020-01-30,Extreme Fermi surface smearing in a maximally disordered concentrated solid solution,"We show that the Fermi surface can survive the presence of extreme compositional disorder in the equiatomic alloy Ni$_{0.25}$Fe$_{0.25}$Co$_{0.25}$Cr$_{0.25}$. Our high-resolution Compton scattering experiments reveal a Fermi surface which is smeared across a significant fraction of the Brillouin zone (up to 40\% of $\frac{2\pi}{a}$). The extent of this smearing and its variation on and between different sheets of the Fermi surface has been determined, and estimates of the electron mean-free-path and residual resistivity have been made by connecting this smearing with the coherence length of the quasiparticle states.",2001.11416v1 2020-05-12,Superconductivity in Hydrogenated Graphites,"We report transport and magnetization measurements on graphitic materials that have been hydrogenated after being treated with octane. The temperature-dependent electrical resistivity shows anomalies manifested as re-entrant insulator-metal transitions. Below 50 K, the magnetoresistance data shows both antiferromagnetic and ferromagnetic behavior as the magnetic field is decrease or increased, respectively. The system is possibly an unconventional magnetic superconductor. The irreversible behavior observed in the field-cooled vs. the zero-field cooled data for a sufficiently high magnetic field suggests that the system might enter a superconducting state below 50 K. Energy gap data is obtained from nonlocal electric differential conductance measurements. An exciton-based mechanism is likely driving the system to the superconducting state below 50 K, where the gap is divergent. We find that the hydrogenated carbon fiber is a multiple gap system with critical temperatures estimates above room temperature. The temperature dependence of the superconducting gap follows the flat-band energy relationship, with the flat band gap parameter linearly increasing with the temperature above 50 K. Thus, we find that either a magnetic or an electric field can drive this hydrogenated graphitic system to superconducting state below 50 K. In addition, AF spin fluctuations creates pseudo-gap states above 50 K.",2005.05876v1 2020-07-02,Drone swarms in fire suppression activities,"Recent huge technological development of Unmanned Aerial Vehicles (UAVs) can provide breakthrough means of fighting wildland fires. We propose an innovative forest firefighting system based on the use of a swarm of hundreds of UAVs able to generate a continuous flow of extinguishing liquid on the fire front, simulating rain effect. Automatic battery replacement and refilling of the extinguishing liquid ensure the continuity of the action, and fire-resistant materials protect drones exposed to possible high temperatures. We demonstrate the validity of the approach in Mediterranean scrub first computing the critical water flow rate according to the main factors involved in the evolution of a fire, then estimating the number of linear meters of active fire front that can be extinguished depending on the number of drones available and the amount of extinguishing fluid carried. A fire propagation cellular automata model is also employed to study the evolution of the fire. Simulation results suggest that the proposed system can successfully integrate, or in case of low-intensity and limited extent fires completely replace, current forest firefighting techniques.",2007.00883v2 2020-07-29,Energy Transfer to a Stable Donor Suppresses Degradation in Organic Solar Cells,"Despite many advances towards improving the stability of organic photovoltaic devices, environmental degradation under ambient conditions remains a challenging obstacle for future application. Particularly conventional systems employing fullerene derivatives are prone to oxidise under illumination, limiting their applicability. Herein, we report on the environmental stability of the small molecule donor DRCN5T together with the fullerene acceptor PC70BM. We find that this system exhibits exceptional device stability, mainly due to almost constant short-circuit current. By employing ultrafast femtosecond transient absorption spectroscopy we attribute this remarkable stability to two separate mechanisms: 1) DRCN5T exhibits high intrinsic resistance towards external factors, showing no signs of deterioration. 2) The highly sensitive PC70BM is stabilised against degradation by the presence of DRCN5T through ultrafast long-range energy transfer to the donor, rapidly quenching the fullerene excited states which are otherwise precursors for chemical oxidation. We propose that this photoprotective mechanism be utilised to improve the device stability of other systems, including non-fullerene acceptors and ternary blends.",2007.14651v1 2020-10-13,Strong anisotropy of electron-phonon interaction in NbP probed by magnetoacoustic quantum oscillations,"In this study, we report on the observation of de Haas-van Alphen-type quantum oscillations (QO) in the ultrasound velocity of NbP as well as `giant QO' in the ultrasound attenuation in pulsed magnetic fields. The difference of the QO amplitude for different acoustic modes reveals a strong anisotropy of the effective deformation potential, which we estimate to be as high as $9\,\mathrm{eV}$ for certain parts of the Fermi surface. Furthermore, the natural filtering of QO frequencies and the tracing of the individual Landau levels to the quantum limit allows for a more detailed investigation of the Fermi surface of NbP as was previously achieved by means of analyzing QO observed in magnetization or electrical resistivity.",2010.06530v2 2020-10-13,Stacking-engineered ferroelectricity in bilayer boron nitride,"2D ferroelectrics with robust polarization down to atomic thicknesses provide novel building blocks for functional heterostructures. Experimental reports, however, remain scarce because of the requirement of a layered polar crystal. Here, we demonstrate a rational design approach to engineering 2D ferroelectrics from a non-ferroelectric parent compound via employing van der Waals assembly. Parallel-stacked bilayer boron nitride is shown to exhibit out-of-plane electric polarization that reverses depending on the stacking order. The polarization switching is probed via the resistance of an adjacently-stacked graphene sheet. Furthermore, twisting the boron nitride sheets by a small-angle changes the dynamics of switching due to the formation of moir\'e ferroelectricity with staggered polarization. The ferroelectricity persists to room temperature while keeping the high mobility of graphene, paving the way for potential ultrathin nonvolatile memory applications.",2010.06600v2 2020-10-16,Visualizing half-metallic bulk band structure with multiple Weyl cones of the Heusler ferromagnet,"Using a well-focused soft X-ray synchrotron radiation beam, angle-resolved photoelectron spectroscopy was applied to a full-Heusler-type Co$_2$MnGe alloy to elucidate its bulk band structure. A large parabolic band at the Brillouin zone center and several bands that cross the Fermi level near the Brillouin zone boundary were identified in line with the results from first-principles calculations. These Fermi level crossings are ascribed to majority spin bands that are responsible for electron transport with extremely high spin polarization especially along the direction being perpendicular to the interface of magneto-resistive devices. The spectroscopy confirms there is no contribution of the minority spin bands to the Fermi surface, signifying half-metallicity for the alloy. Furthermore, two topological Weyl cones with band crossing points were identified around the $X$ point, yielding the conclusion that Co$_2$MnGe could exhibit topologically meaningful behavior such as large anomalous Hall and Nernst effects driven by the Berry flux in its half-metallic band structure.",2010.08415v1 2020-10-27,Superconductivity and Fermi Surface Nesting in the Candidate Dirac Semimetal NbC,"We report the synthesis of single-crystal NbC, a transition metal carbide with various unusual properties. Transport, magnetic susceptibility, and specific heat measurements demonstrate that NbC is a conventional superconductor with a superconducting transition temperature ($T_c$) of 11.5 K. Our theoretical calculations show that NbC is a type-II Dirac semimetal with strong Fermi surface nesting, which is supported by our ARPES measurement results. We also observed the superconducting gaps of NbC using angle-resolved photoemission spectroscopy (ARPES) and found some unconventional behaviors. These intriguing superconducting and topological properties, combined with the high corrosion resistance, make NbC an ideal platform for both fundamental research and device applications.",2010.14259v2 2020-11-02,Phase field predictions of microscopic fracture and R-curve behaviour of fibre-reinforced composites,"We present a computational framework to explore the effect of microstructure and constituent properties upon the fracture toughness of fibre-reinforced polymer composites. To capture microscopic matrix cracking and fibre-matrix debonding, the framework couples the phase field fracture method and a cohesive zone model in the context of the finite element method. Virtual single-notched three point bending tests are conducted. The actual microstructure of the composite is simulated by an embedded cell in the fracture process zone, while the remaining area is homogenised to be an anisotropic elastic solid. A detailed comparison of the predicted results with experimental observations reveals that it is possible to accurately capture the crack path, interface debonding and load versus displacement response. The sensitivity of the crack growth resistance curve (R-curve) to the matrix fracture toughness and the fibre-matrix interface properties is determined. The influence of porosity upon the R-curve of fibre-reinforced composites is also explored, revealing a stabler response with increasing void volume fraction. These results shed light into microscopic fracture mechanisms and set the basis for efficient design of high fracture toughness composites.",2011.00779v1 2020-11-10,Rebound suppression of a droplet impact on a supersolvophobic surface by a small amount of polymer additives,"A small amount of polymer dissolved in a droplet suppresses droplet rebound when it impinges on a supersolvophobic surface. This work investigates impacting dynamics of a droplet of dilute polymer solution depending on the molecular weight and the concentration of the polymer by using multi-body dissipative particle dynamics simulations. Either the longer polymer or the high polymer concentration suppresses rebound of a droplet although its shear viscosity and the liquid-vapor surface tension are not different from those of a pure solvent droplet. We found a new mechanism of the anti-rebound in which the resistance is applied against the hopping motion, while behavior of the non-rebounding droplet at the earlier spreading and retraction stages is same as for the rebounding droplets. Two polymer contributions to reducing the rebound tendency are quantitatively analyzed: the alteration of the substrate wettability by the polymer adsorption and the polymer elongation force.",2011.05086v1 2020-12-03,Optical and Hidden Transport Properties of BaFe$_{1.91}$Ni$_{0.09}$As$_{2}$ Film,"Optical spectroscopy was used to study the electrodynamics and hidden transport properties of a BaFe$_{1.91}$Ni$_{0.09}$As$_{2}$ thin superconducting film. We analyzed the normal state data using a Drude-Lorentz model with two Drude components: one narrow ($D_1$) and another broad one ($D_2$). In the superconducting state, two gaps with $2\Delta _{0}^{(2)}/k_BT_c=1.9$--2.0 and $2\Delta _{0}^{(1)}/k_BT_c=4.0$--4.3 are formed from the narrow component $D_1$ while the broad component $D_2$ remains ungapped. The calculated total DC resistivity of the film and the low-temperature scattering rate for the narrow Drude component show a hidden Fermi-liquid behavior. The change of total electron-boson coupling ($\lambda_{tot}$) and representative energy ($\Omega_{0}$) in the normal state with respect to the superconducting state is typical of other iron-based materials as well as high-temperature superconducting (HTSC) cuprates.",2012.01962v1 2020-12-08,Phonon modes contribution in thermal rectification in graphene-C3B junction: A molecular dynamics study,"In this work using non-equilibrium molecular dynamics simulation we implement a series of simulation under positive and negative temperature gradient in order to investigate the thermal rectification in the graphene C3B junction GCB. The dependence of thermal rectification on temperature difference between the hot and the cold baths is obtained. The important quantity that we present here is the inplanes and out of plane phonon modes contribution in the thermal rectification. We see that the Y mode has high and positive thermal rectification while that the X and Z modes have small and negative thermal rectifications. Thermal rectification for Y mode increases sharply beyond T 30 K to 150 but for X and Z modes decrease slowly by increasing T Our results show that Y mode has major role in the thermal rectification Moreover the underlying mechanisms that leads to the thermal rectification and also Kapitza resistance at the interface are studied via the phonon density of states DOS",2012.04363v1 2021-04-14,Lack of Fusion in Additive Manufacturing: Defect or Asset?,"Rapid cooling rates and stochastic interactions between the heat source and feedstock in additive manufacturing (AM) result in strong anisotropy and process-induced defects deteriorating the tensile ductility and fatigue resistance of printed parts. We show that by deliberately introducing a high density of lack of fusion (LoF) defects, a processing regime that has been avoided so far, followed by pressure assisted heat treatment, we can print Ti-6Al-4V with reduced texture and exceptional properties surpassing that of wrought, cast, forged, annealed, and solution-treated and aged counterparts. Such improvement is achieved through the formation of low aspect ratio {\alpha}-grains around LoF defects upon healing, surrounded by {\alpha}-laths. This occurrence is attributed to surface energy reduction and recrystallization events taking place during healing of LoF defects. Our approach to design duplex microstructures is applicable to a wide range of AM processes and alloys and can be used in the design of damage tolerant microstructures.",2104.07014v1 2021-04-21,Electrically detected paramagnetic resonance in Ag-paint coated DPPH,"We describe a simple experimental method to detect electron paramagnetic resonance (EPR) in polycrystalline 2,2-diphenyl-1-picrylhydrazyl (DPPH) sample, the standard g-marker for EPR spectroscopy, without using a cavity resonator or a prefabricated waveguide. It is shown that microwave(MW) current injected into a layer of silver paint coated on an insulating DPPH sample is able to excite the paramagnetic resonance in DPPH. As the applied dc magnetic field H is swept, the high-frequency resistance of the Ag-paint layer, measured at room temperature with a single port impedance analyzer in the MW frequency range 1 to 2.5 GHz, exhibits a sharp peak at a critical value of the dc field (H = Hres) while the reactance exhibits a dispersion-like behavior around the same field value for a given frequency. Hres increases linearly with the frequency of MW current. We interpret the observed features in the impedance to EPR in DPPH driven by the Oersted magnetic field arising from the MW current in the Ag-paint layer. We also confirm the occurrence of EPR in DPPH independently using a coplanar waveguide-based broadband technique. This technique has the potential to investigate other EPR active inorganic and organic compounds.",2104.10794v1 2021-05-26,Theoretical study for 3D quantum Hall effect in a periodic electron system,"The exsitance of three-dimensional Hall effect (3DQHE) due to spontaneous Fermi surface instabilities in strong magnetic field was proposed decades ago, and has stimulated recent progress in experiments. The reports in recent experiments show that the Hall plateaus and vanishing transverse magneto-resistivities (TMRs) (which are two main signatures of 3DQHE) are not easy to be observed in natural materials. And two main different explanations of the slow varying slope like Hall plateaus and non-vanishing TMRs (which can be called as quasi-quantized Hall effect (QQHE)) have been proposed. By studying the magneto-transport with a simple effective periodic 3D system, we show how 3DQHE can be achieved in certain parameter regimes at first. We find two new mechanisms that may give rise to QQHE. One mechanism is the ""low"" Fermi energy effect, and the other is the ""strong"" impurity effect. Our studies also proved that the artificial superlattice is an ideal platform for realizing 3DQHE with high layer barrier periodic potential.",2105.12461v2 2021-06-09,"The extended diffusive Sachdev-Ye-Kitaev model as a sort of ""strange metal""","The 0+1-d Sachdev-Ye-Kitaev (SYK) fermionic model attracts nowadays a wide spread interest of the Condensed Matter community, as a benchmark toy model for strong electron correlation and non Fermi Liquid behavior. It is exactly solvable in the infrared limit and reproduces the linear dependence of the resistivity on temperature T, in linear response, typical of the strange metal phase of High Temperature Superconducting (HTS) materials. The breaking of its conformal symmetry requires ultraviolet corrections for a faithful description of its pseudo Goldstone Modes. Extension of the model to higher space dimension includes a local U(1) phase generating collective bosonic excitations driven by the additional ultraviolet contribution to the action. These excitations are studied here, in a temperature window of incoherent dynamics in which the expected chaotic regime has not yet taken over. We identify them as neutral diffusive energy excitations with temperature dependent lifetime h / k_B T. They provide thermalization of the system and contribute to the T dependence of the transport coefficients. The linear unbound T increase of particle current is confirmed by our hydrodynamic modelization. A quantum liquid in interaction with this system would become a Marginal Fermi Liquid.",2106.05383v2 2021-06-15,Charge Carrier Transport in Iron Pyrite Thin Films: Disorder Induced Variable Range Hopping,"The origin of p-type conductivity and the mechanism responsible for low carrier mobility was investigated in pyrite (FeS2) thin films. Temperature dependent resistivity measurements were performed on polycrystalline and nanostructured thin films prepared by three different methods. Films have a high hole density and low mobility regardless of the method used for their preparation. The charge transport mechanism is determined to be nearest neighbour hopping (NNH) at near room temperature with Mott-type variable range hopping (VRH) of holes via localized states occurring at lower temperatures. Density functional theory (DFT) predicts that sulfur vacancy induced localized defect states will be situated within the band gap with the charge remaining localized around the defect. The data indicate that the electronic properties including hopping transport in pyrite thin films can be correlated to sulfur vacancy related defect. The results provide insights on electronic properties of pyrite thin films and its implications for charge transport",2106.08401v2 2021-06-24,Epitaxial growth of Ruddlesden-Popper neodymium nickelates Nd$_{n+1}$Ni$_{n}$O$_{3n+1}$ (${n}$ = 1-5),"A series of Ruddlesden-Popper nickelates, Nd$_{n+1}$Ni$_{n}$O$_{3n+1}$ (${n}$ = 1-5), have been stabilized in thin film form using reactive molecular-beam epitaxy. High crystalline quality has been verified by X-ray diffraction and scanning transmission electron microscopy. X-ray photoelectron spectroscopy indicates the ${n}$-dependent valence states of nickel in these compounds. Metal-insulator transitions show clear ${n}$ dependence for intermediate members (${n}$ = 3-5), and the low-temperature resistivities of which show logarithmic dependence, resembling the Kondo-scattering as observed in the parent compounds of superconducting infinite-layer nickelates.",2106.12941v1 2021-07-28,Narrow-gap semiconducting behavior in antiferromagnetic Eu$_{11}$InSb$_9$,"Here we investigate the thermodynamic and electronic properties of Eu$_{11}$InSb$_9$ single crystals. Electrical transport data show that Eu$_{11}$InSb$_9$ has a semiconducting ground state with a relatively narrow band gap of $320$~meV. Magnetic susceptibility data reveal antiferromagnetic order at low temperatures, whereas ferromagnetic interactions dominate at high temperature. Specific heat, magnetic susceptibility, and electrical resistivity measurements reveal three phase transitions at $T_{N1}=9.3$~K, $T_{N2} =8.3$~K, and $T_{N3} =4.3$~K. Unlike Eu$_{5}$In$_{2}$Sb$_6$, a related europium-containing Zintl compound, no colossal magnetoresistance (CMR) is observed in Eu$_{11}$InSb$_9$. We attribute the absence of CMR to the smaller carrier density and the larger distance between Eu ions and In-Sb polyhedra in Eu$_{11}$InSb$_9$. Our results indicate that Eu$_{11}$InSb$_9$ has potential applications as a thermoelectric material through doping or as a long-wavelength detector due to its narrow gap.",2107.13145v1 2021-08-04,Theory of Huge Thermoelectric Effect Based on Magnon Drag Mechanism: Application to Thin-Film Heusler Alloy,"To understand the unexpectedly high thermoelectric performance observed in the thin-film Heusler alloy Fe$_2$V$_{0.8}$W$_{0.2}$Al, we study the magnon drag effect, generated by the tungsten based impurity band, as a possible source of this enhancement, in analogy to the phonon drag observed in FeSb$_2$. Assuming that the thin-film Heusler alloy has a conduction band integrating with the impurity band, originated by the tungsten substitution, we derive the electrical conductivity $L_{11}$ based on the self-consistent t-matrix approximation and the thermoelectric conductivity $L_{12}$ due to magnon drag, based on the linear response theory, and estimate the temperature dependent electrical resistivity, Seebeck coefficient and power factor. Finally, we compare the theoretical results with the experimental results of the thin-film Heusler alloy to show that the origin of the exceptional thermoelectric properties is likely to be due to the magnon drag related with the tungsten-based impurity band.",2108.01880v1 2021-08-10,Nature of electrons from oxygen vacancies and polar catastrophe at LaAlO3/SrTiO3 interfaces,"The relative significance of quantum conductivity correction and magnetic nature of electrons in understanding the intriguing low-temperature resistivity minimum and negative magnetoresistance of the two-dimensional electron gas at LaAlO3/SrTiO3 interfaces has been a long outstanding issue since its discovery. Here we report a comparative magnetotransport study on amorphous and oxygen-annealed crystalline LaAlO3/SrTiO3 heterostructures at a relatively high-temperature range, where the orbital scattering is largely suppressed by thermal fluctuations. Despite of a predominantly negative out-of-plane magnetoresistance effect for both, the magnetotransport is isotropic for amorphous LaAlO3/SrTiO3 while strongly anisotropic and well falls into a two-dimensional quantum correction frame for annealed crystalline LaAlO3/SrTiO3. These results clearly indicate that a large portion of electrons from oxygen vacancies are localized at low temperatures, serving as magnetic centers, while the electrons from the polar field are only weakly localized due to constructive interference between time-reversed electron paths in the clean limit and no signature of magnetic nature is visible.",2108.04532v1 2021-08-19,"Chemomechanics: friend or foe of the ""AND problem"" of solid-state batteries?","Solid electrolytes are widely considered as the enabler of lithium metal anodes for safe, durable, and high energy density rechargeable lithium-ion batteries. Despite the promise, failure mechanisms associated with solid-state batteries are not well-established, largely due to limited understanding of the chemomechanical factors governing them. We focus on the recent developments in understanding solid-state aspects including the effects of mechanical stresses, constitutive relations, fracture, and void formation, and outline the gaps in the literature. We also provide an overview of the manufacturing and processing of solid-state batteries in relation to chemomechanics. The gaps identified provide concrete directions towards the rational design and development of failure-resistant solid-state batteries.",2108.10150v2 2021-09-01,Electrical switching of antiferromagnetic CoO | Pt across the Néel temperature,"One of the most important challenges in antiferromagnetic spintronics is the read-out of the N\'eel vector state. High current densities up to 10$^8$ Acm$^{-2}$ used in the electrical switching experiments cause notorious difficulty in distinguishing between magnetic and thermal origins of the electrical signals. To overcome this problem, we present a temperature dependence study of the transverse resistance changes in the switching experiment with CoO|Pt devices. We demonstrate the possibility to extract a pattern of spin Hall magnetoresistance for current pulses density of $5 \times 10^7$ Acm$^{-2}$ that is present only below the N\'eel temperature and does not follow a trend expected for thermal effects. This is the compelling evidence for the magnetic origin of the signal, which is observed using purely electrical techniques. We confirm these findings by complementary experiments in an external magnetic field. Such an approach can allow determining the optimal conditions for switching antiferromagnets and be very valuable when no imaging techniques can be applied to verify the origin of the electrical signal.",2109.00293v2 2021-09-22,Dynamic Behaviors and Training Effects in TiN/Ti/HfO$_x$/TiN Nanolayered Memristors with Controllable Quantized Conductance States: Implications for Quantum and Neuromorphic Computing Devices,"Controllable quantized conductance states of TiN/Ti/HfO$_x$/TiN memristors are realized with great precision through a pulse-mode reset procedure, assisted with analytical differentiation of the condition of the set procedure, which involves critical monitoring of the measured bias voltage. An intriguing training effect that leads to faster switching of the states is also observed during the operation. Detailed analyses on the low- and high-resistance states under different compliance currents reveal a complete picture of the structural evolution and dynamic behaviors of the conductive filament in the HfO$_x$ layer. This study provides a closer inspection on the quantum-level manipulation of nanoscale atomic configurations in the memristors, which helps to develop essential knowledge about the design and fabrication of the future memristor-based quantum devices and neuromorphic computing devices.",2109.10783v1 2021-09-27,Strongly electron-correlated semimetal RuI$_3$ with a layered honeycomb structure,"A polymorph of RuI$_3$ synthesized under high pressure was found to have a two-layered honeycomb structure. The resistivity of RuI$_3$ exhibits a semimetallic behavior, in contrast to insulating properties in $\alpha$-RuCl$_3$. In addition, Pauli paramagnetic behavior was observed in the temperature dependence of a magnetic susceptibility and a nuclear spin-lattice relaxation rate 1/$T_1$. The band structure calculations indicate that contribution of the I 5$p$ components to the low-energy $t_\mathrm{2g}$ bands effectively decreases Coulomb repulsion, leading to semimetallic properties. The physical properties also suggest strong electron correlations in RuI$_3$.",2109.12864v2 2021-10-12,Single-component superconducting state in UTe2 at 2 K,"UTe2 is a newly-discovered unconventional superconductor wherein multicomponent topological superconductivity is anticipated based on the presence of two superconducting transitions and time-reversal symmetry breaking in the superconducting state. The observation of two superconducting transitions, however, remains controversial. Here we demonstrate that UTe2 single crystals displaying an optimal superconducting transition temperature at 2 K exhibit a single transition and remarkably high quality supported by their small residual heat capacity in the superconducting state and large residual resistance ratio. Our results shed light on the intrinsic superconducting properties of UTe2 and bring into question whether UTe2 is a multicomponent superconductor at ambient pressure.",2110.06200v1 2021-10-13,Large-Gap Quantum Spin Hall State and Temperature-Induced Lifshitz Transition in Bi4Br4,"Searching for new quantum spin Hall insulators with large fully opened energy gap to overcome the thermal disturbance at room temperature has attracted tremendous attention due to the one-dimensional (1D) spin-momentum locked topological edge states serving as dissipationless channels for the practical applications in low consumption electronics and high performance spintronics. Here, we report the investigation of topological nature of monolayer Bi4Br4 by the techniques of scanning tunneling microscopy and angle-resolved photoemission spectroscopy (ARPES). The topological non-triviality of 1D edge state integrals within the large bulk energy gap (~ 0.2 eV) is revealed by the first-principle calculations. The ARPES measurements at different temperature show a temperature-induced Lifshitz transition, corresponding to the resistivity anomaly caused by the shift of chemical potential. The connection between the emergency of superconductivity and the Lifshitz transition is discussed.",2110.06658v1 2021-11-09,Weak antilocalization and Shubnikov-de Haas oscillations in CaCuSb single crystal,"Quantum oscillations in both linear and Hall resistivities and weak antilocalization (WAL) are barely observed in bulk single crystals. Here we report the transport properties of a CaCuSb single crystal that crystallizes in the hexagonal crystal structure. The magnetotransport studies reveal WAL and Shubnikov-de Haas (SdH) quantum oscillations with a unique frequency at 314 T. A cusp-like behavior in the low field regime of magnetotransport for J // (ab)-plane and B // [0001] confirms the WAL in CaCuSb. Angular-dependent normalized magnetoconductance and SdH oscillations studies reveal that the observed phenomena originate from the 2D transport channels. The high magnetic field (up to 45 T) experiments demonstrate plateau-like features in the Hall measurements. The first-principles calculations unfold that CaCuSb is a non-topological semimetal with dominant hole carries at the Fermi level. Our study reveals that CaCuSb is a promising candidate to explore the quasi-2D quantum transport phenomenon in the transition metal pnictide materials.",2111.04996v1 2021-11-29,High-Speed Light Focusing through Scattering Medium by Cooperatively Accelerated Genetic Algorithm,"We develop an accelerated Genetic Algorithm (GA) system constructed by the cooperation of field-programmable gate array (FPGA) and optimized parameters of the GA. We found the enhanced decay of mutation rate makes convergence of the GA much faster, enabling the parameter-induced acceleration of the GA. Furthermore, the accelerated configuration of the GA is programmed in FPGA to boost processing speed at the hardware level without external computation devices. This system has ability to focus light through scattering medium within 4 seconds with robust noise resistance and stable repetition performance, which could be further reduced to millisecond level with advanced board configuration. This study solves the long-term limitation of the GA, it promotes the applications of the GA in dynamic scattering mediums, with the capability to tackle wavefront shaping in biological material.",2111.14916v1 2021-12-01,Atomistic simulations of twin boundary effect on the crack growth behaviour in BCC Fe,"In this paper, the effect of twin boundaries on the crack growth behaviour of single crystal BCC Fe has been investigated using molecular dynamics simulations. The growth of an atomically sharp crack with an orientation of (111)$<$110$>$ (crack plane/crack front) has been studied under mode-I loading at constant strain rate. In order to study the influence of twin boundaries on the crack growth behaviour, single and multiple twin boundaries were introduced perpendicular to crack growth direction. The results indicate that the (111)$<$110$>$ crack in single crystal BCC Fe grows in brittle manner. However, following the introduction of twin boundaries, a noticeable plastic deformation has been observed at the crack tip. Further, increasing the number of twin boundaries increased the amount of plastic deformation leading to better crack resistance and high failure strains. Finally, an interesting relationship has been observed between the crack growth rate and flow stress.",2112.00354v1 2022-01-10,Phase Boundary Segregation in Multicomponent Alloys: A Diffuse-Interface Thermodynamic Model,"Microalloying elements tend to segregate to the matrix-precipitate phase boundaries to reduce the interfacial energy. The segregation mechanism is emerging as a novel design strategy for developing precipitation-hardened alloys with significantly improved coarsening resistance for high temperature applications. In this paper, we report a nanoscopic diffuse-interface thermodynamic model that describes multicomponent segregation behavior in two-phase substitutional alloys. Following classical approaches for grain boundaries, we employ the regular solution thermodynamics to establish segregation isotherms. We show that the model recovers the Guttmann multicomponent isotherm describing local interfacial concentrations, and the generalized Gibbs adsorption isotherm that governs the total solute excess and interfacial energy. A variety of multicomponent segregation behaviors are demonstrated for a model two-phase quaternary alloy. The nature of interfacial parameters and the resulting analytic solutions make the model amenable for parameterization and comparison with atomistic calculations and experimental characterizations.",2201.03117v1 2022-03-09,Magnetotransport due to conductivity fluctuations in non-magnetic ZrTe2 nanoplates,"Transition metal dichalcogenides with nontrivial band structures exhibit various fascinating physical properties and have sparked intensively research interest. Here, we performed systematic magnetotransport measurements on mechanical exfoliation prepared ZrTe2 nanoplates. We revealed that the negative longitudinal magnetoresistivity observed at high field region in the presence of parallel electric and magnetic fields could stem from the conductivity fluctuations due to the excess Zr in the nanoplates. In addition, the parametric plot, the planar Hall resistivity as function of the in-plane anisotropic magnetoresistivity, has an ellipse-shaped pattern with shifted orbital center, which further strengthen the evidence for the conductivity fluctuations. Our work provides some useful insights into transport phenomena in topological materials.",2203.04486v1 2022-03-11,Ultrafast intrinsic optical-to-electrical conversion dynamics in graphene photodetector,"Optical-to-electrical (O-E) conversion in graphene is a central phenomenon for realizing anticipated ultrafast and low-power-consumption information technologies. However, revealing its mechanism and intrinsic time scale require uncharted terahertz (THz) electronics and device architectures. Here, we succeeded in resolving O-E conversion processes in high-quality graphene by on-chip electrical readout of ultrafast photothermoelectric current. By suppressing the RC time constant using a resistive zinc oxide top gate, we constructed a gate-tunable graphene photodetector with a bandwidth of up to 220 GHz. By measuring nonlocal photocurrent dynamics, we found that the photocurrent extraction from the electrode is instantaneous without a measurable carrier transit time across several-micrometer-long graphene, following the Shockley-Ramo theorem. The time for photocurrent generation is exceptionally tunable from immediate to > 4 ps, and its origin is identified as Fermi-level-dependent intraband carrier-carrier scattering. Our results bridge the gap between ultrafast optical science and device engineering, accelerating ultrafast graphene optoelectronic applications.",2203.05752v1 2022-03-14,Little-Parks like oscillations in lightly doped cuprate superconductors,"Understanding the rich and competing electronic orders in cuprate superconductors may provide important insight into the mechanism of high-temperature superconductivity. Here, by measuring Bi2Sr2CaCu2O8+x in the extremely underdoped regime, we obtain evidence for a distinct type of ordering, which manifests itself as resistance oscillations at low magnetic fields (<10 T) and at temperatures around the superconducting transition. By tuning the doping level p continuously, we reveal that these low-field oscillations occur only when p<0.1. The oscillation amplitude increases with decreasing p but the oscillation period stays almost constant. We show that these low-field oscillations can be well described by assuming a periodic superconducting structure with a mesh size of about 50 nm. Such a charge order, which is distinctly different from the well-established charge density wave and pair density wave, seems to be an unexpected piece of the puzzle on the correlated physics in cuprates.",2203.06971v1 2022-03-25,Hydrodynamic Interactions Between Charged and Uncharged Brownian Colloids at a Fluid-Fluid Interface,"Hypothesis: The collective dynamics and self-assembly of colloids floating at a fluid/fluid interface is a balance between deterministic lateral interaction forces, viscous resistance to colloid motion along the surface and thermal (Brownian) fluctuations. As the colloid size decreases, thermal forces become important and can affect the self assembly into ordered patterns and crystal structures that are the starting point for various materials applications. Numerics: Langevin dynamic simulations involving two particles straddling a liquid/liquid interface with a high viscosity contrast are presented to describe the lateral interfacial assembly of particles in Brownian and non-Brownian dominated regimes. These simulations incorporate capillary attraction, electrostatic repulsion, thermal fluctuations and HI between particles (including the effect of the particle immersion depth). Simulation results are presented for neutrally wetted particles which form a contact angle of 90 degrees at the interface. Findings: Clustering, fractal growth and particle ordering are observed at critically large values of the Pe numbers, while smaller Pe numbers exhibit higher probabilities of yielding states in which particles remain uncorrelated in space and more widely separated.",2203.13925v2 2022-04-02,Upscaling of a reaction-diffusion-convection problem with exploding non-linear drift,"We study a reaction-diffusion-convection problem with nonlinear drift posed in a domain with periodically arranged obstacles. The non-linearity in the drift is linked to the hydrodynamic limit of a totally asymmetric simple exclusion process (TASEP) governing a population of interacting particles crossing a domain with obstacle. Because of the imposed large drift scaling, this nonlinearity is expected to explode in the limit of a vanishing scaling parameter. As main working techniques, we employ two-scale formal homogenization asymptotics with drift to derive the corresponding upscaled model equations as well as the structure of the effective transport tensors. Finally, we use Schauder's fixed point theorem as well as monotonicity arguments to study the weak solvability of the upscaled model posed in an unbounded domain. This study wants to contribute with theoretical understanding needed when designing thin composite materials that are resistant to high velocity impacts.",2204.00931v1 2022-06-01,Charge density wave and superconductivity in 6R-TaS2,"The layered transition metal dichalcogenide compounds 1T-TaS2 and 4H-TaS2 are well known for their exotic properties, which include charge density wave, superconductivity, Mott transition, etc., and lately quantum spin liquid. Here, we report the magnetic, transport and transmission electron microscopy study of the charge density wave and superconductivity in 6R-TaS2 which is a relatively less studied polymorph of this dichalcogenide TaS2. Our high temperature electron microscopy reveals multiple charge density wave transitions between room temperature and 650K. Magnetization, and the electrical resistivity measurements in the temperature range of 2-400 K reveal that 6R-TaS2 undergoes a charge density wave transition around 305 K and is followed by a transition to a superconducting state around 3.5 K. The low temperature specific heat measurement exhibits anomaly associated with the superconducting transition around 2.4 K. The estimated Ginzburg Landau parameter suggests that this compound lies at the extreme limit of type-II superconductivity.",2206.00281v3 2022-06-03,Effects of charge dopants in quantum spin Hall materials,"Semiconductors' sensitivity to electrostatic gating and doping accounts for their widespread use in information communication and new energy technologies. It is demonstrated quantitatively and with no adjustable parameters that the presence of paramagnetic acceptor dopants elucidates a variety of hitherto puzzling properties of two-dimensional topological semiconductors at the topological phase transition and in the regime of the quantum spin Hall effect. The concepts of charge correlation, Coulomb gap, exchange interaction between conducting electrons and holes localized on acceptors, strong coupling limit of the Kondo effect, and bound magnetic polaron explain a short topological protection length, high hole mobilities compared with electron mobilities, and different temperature dependence of the spin Hall resistance in HgTe and (Hg,Mn)Te quantum wells.",2206.01613v3 2022-06-02,Modeling Defect-Level Switching for Highly-Nonlinear and Hysteretic Electronic Devices,"Many semiconductors feature defects with charge state transition levels that can switch due to structure changes following defect ionization: we call this defect-level switching (DLS). For example, DX centers in III-V compounds, and oxygen vacancies in ZnO, can switch between deep and shallow donor configurations, and these bistable dynamics are responsible for persistent photoconductivity. We recently demonstrated highly-nonlinear, hysteretic, two-terminal electronic devices using DLS in CdS [H. Yin, A. Kumar, J.M. LeBeau, and R. Jaramillo, Phys. Rev. Applied 15, 014014 (2021).] The resulting devices operate without mass transport, and in the opposite sense to most resistive switches: they are in a high-conductivity state at equilibrium, and switch to a low-conductivity state at forward bias. Although DLS uses the same defect transitions that are responsible for persistent photoconductivity, DLS devices operate without light and can be orders-of-magnitude faster due to exponential tuning of transition rates with voltage. In this work we use theory and numerical simulation to explore the design space of DLS devices, emphasizing the tradeoff between speed and on/off ratio. Our results will be useful to guide future applications of these unusual devices.",2206.04108v1 2022-10-14,The Electrical Property of Large Few Layer Graphene Flakes Obtained by Microwaves Assisted Exfoliation of Expanded Graphite,"Few layer graphene (FLG) was synthesized by $\mu$-wave assisted exfoliation of expanded graphite in toluene with an overall yield from c.a. 7% to 20%. A significant difference in the absorption of $\mu$-waves by the expanded graphite and toluene allowed a rapid heating of the medium. The number of FLG sheets varies from 3 to 12, while the lateral size of the sheets exceeds few $\mu$ms. The obtained FLG exhibits very low resistance with average value of 1.6 k$\Omega$ (500 $\Omega$ minimum) which is comparable to that of high quality graphenes synthesized by CVD methods, and lower than numbers of exfoliated graphenes.",2210.07627v1 2022-10-26,Superior damage tolerance of fish skins,"Skin is the largest organ of many animals. Its protective function against hostile environments and predatorial attack makes high mechanical strength a vital characteristic. Here, we measured the mechanical properties of bass fish skins and found that fish skins are highly ductile with a rupture strain of up to 30-40% and a rupture strength of 10-15 MPa. The fish skins exhibit a strain-stiffening behavior. Stretching can effectively eliminate the stress concentrations near the pre-existing holes and edge notches, suggesting that the skins are highly damage tolerant. Our measurement determined a flaw-insensitivity length of several millimeters, which exceeds that of most engineering materials. The strain-stiffening and damage tolerance of fish skins are explained by an agent-based model of collagen network in which the load-bearing collagen microfibers assembled from nanofibrils undergo straightening and reorientation upon stretching. Our study inspires development of artificial skins that are thin, flexible, but highly fracture-resistant and widely applicable in soft robots.",2210.14651v1 2022-10-29,Magnetotransport Properties and Fermi Surface Topology of Nodal line Semimetal InBi,"In the present study, we have discussed the up-turn behavior in the resistivity pattern of the topological nodal line semimetal InBi. We argued that such nature could be generalized with a mathematical model, that can be applied to any compounds exhibiting similar behavior. The extremely high magnetoresistance (XMR) has also been explained by the carrier compensation in the compound, estimated from the Hall conductivity. Moreover, from the study of Subhnikov-de Haas (SdH) oscillation and density functional theory (DFT), we obtained the complete three-dimensional (3D) Fermi surface topology of the compound InBi. A detailed understanding of carriers' behavior has been discussed using those studies. We have also unfurled the topology of each electron and hole pocket and its possible modulation with electron and hole doping.",2210.16527v1 2022-11-30,"Mixed Valence Pseudobrookite Al$_{1.75}$Ti$_{1.25}$O$_5$: High Temperature Phase Transitions, Magnetism and Resistivity","Dark blue single crystals of Al$_{1.75}^{3+}$ Ti$_{1.0}^{4+}$ Ti$_{0.25}^{3+}$O$_5$ were grown with a novel synthesis method based on the reaction of a Ti3+/Ti4+ containing langbeinite melt and Al$_2$O$_3$. The obtained needles crystallize in the pseudobrookite structure and undergo two reversible phase transitions from orthorhombic Cmcm to C2/m first and subsequently to C2 symmetry. Like the known aluminum titanate pseudobrookites, anistropic thermal expansion is observed. The temperature evolution of the crystal structure reveals some insights into the mechanism leading to the decomposition of the Al$_{1.75}$Ti$_{1.25}$O$_5$ above 725$^\circ$C. The magnetic and electrical properties are discussed and compared to other reported aluminum titanate pseudobrookites.",2211.17252v2 2022-12-14,Study of the V$_2^0$ state in neutron-irradiated silicon using photon-absorption measurements,"Pieces of $n$-type silicon with 3.5 k$\Omega \cdot $cm resistivity have been irradiated by reactor neutrons to fluences of (1, 5 and 10) $\times 10^{16}$ cm$^{-2}$. Using light-transmission measurements, the absorption coefficients have been determined for photon energies, $E_\gamma $, between 0.62 and 1.30 eV for the samples as irradiated and after 15 min isochronal annealing with temperatures between 80{\deg}C and 330{\deg}C. The radiation-induced absorption coefficient, $\alpha_\mathit{irr}$, has been obtained by subtracting the absorption coefficient for non-irradiated silicon. The $E_\gamma $-dependence of $\alpha_\mathit{irr}$ shows a resonance peak, which is ascribed to the neutral divacancy, V$_2^0$, sitting on a background, and $\alpha_\mathit{irr} (E_\gamma )$ is fitted by a Breit-Wigner line shape on a parameterized background. It is found that at an annealing temperature of 210{\deg}C the V$_2^0$ intensity is reduced by a factor 2, and that at the meV level, the position and the width of the fitted Breit-Wigner do not change with irradiation dose and annealing.",2212.07320v2 2023-01-18,Schramm-Loewner evolution in 2d rigidity percolation,"Amorphous solids may resist external deformation such as shear or compression while they do not present any long-range translational order or symmetry at the microscopic scale. Yet, it was recently discovered that, when they become rigid, such materials acquire a high degree of symmetry hidden in the disorder fluctuations: their microstructure becomes statistically conformally invariant. In this Letter we exploit this finding to characterise the universality class of central-force rigidity percolation (RP), using Schramm-Loewner Evolution (SLE) theory. We provide numerical evidences that the interfaces of the mechanically stable structures (rigid clusters), at the rigidification transition, are consistently described by SLE$_\kappa$, showing that this powerful framework can be applied to a mechanical percolation transition. Using well-known relations between different SLE observables and the universal diffusion constant $\kappa$, we obtain the estimation $\kappa\sim2.9$ for central-force RP. This value is consistent, through relations coming from conformal field theory, with previously measured values for the clusters' fractal dimension $D_f$ and correlation length exponent $\nu$, providing new, non-trivial relations between critical exponents for RP. These findings open the way to a fine understanding of the microstructure in other important classes of rigidity and jamming transitions.",2301.07614v2 2023-01-26,3D-imaging of Printed Nanostructured Networks using High-resolution FIB-SEM Nanotomography,"Networks of solution-processed nanomaterials are important for multiple applications in electronics, sensing and energy storage/generation. While it is known that network morphology plays a dominant role in determining the physical properties of printed networks, it remains difficult to quantify network structure. Here, we utilise FIB-SEM nanotomography to characterise the morphology of nanostructured networks. Nanometer-resolution 3D-images were obtained from printed networks of graphene nanosheets of various sizes, as well as networks of WS2 nanosheets, silver nanosheets and silver nanowires. Important morphological characteristics, including network porosity, tortuosity, pore dimensions and nanosheet orientation were extracted and linked to network resistivity. By extending this technique to interrogate the structure and interfaces within vertical printed heterostacks, we demonstrate the potential of this technique for device characterisation and optimisation.",2301.11046v1 2023-03-08,Optical rogue waves in spheroids of tumor cells,"Rogue waves are intense and unexpected wavepackets ubiquitous in complex systems. In optics, they are promising as robust and noise-resistant beams for probing and manipulating the underlying material. Localizing large optical power is crucial especially in biomedical systems, where, however, extremely intense beams have not yet been observed. We here discover that tumor-cell spheroids manifest optical rogue waves when illuminated by randomly modulated laser beams. The intensity of light transmitted through bio-printed three-dimensional tumor models follows a signature Weibull statistical distribution, where extreme events correspond to spatially-localized optical modes propagating within the cell network. Experiments varying the input beam power and size indicate the rogue waves have a nonlinear origin. We show these optical filaments form high-transmission channels with enhanced transmission. They deliver large optical power through the tumor spheroid, which can be exploited to achieve a local temperature increase controlled by the input wave shape. Our findings shed new light on optical propagation in biological aggregates and demonstrate how extreme event formation allows light concentration in deep tissues, paving the way to using rogue waves in biomedical applications such as light-activated therapies.",2303.04553v1 2023-04-28,Experimental observation of metallic states with different dimensionality in a quasi-1D charge density wave compound,"TaTe$_4$ is a quasi-1D tetrachalcogenide that exhibits a CDW instability caused by a periodic lattice distortion. Recently, pressure-induced superconductivity has been achieved in this compound, revealing a competition between these different ground states and making TaTe$_4$ very interesting for fundamental studies. Although TaTe$_4$ exhibits CDW ordering below 475 K, transport experiments have reported metallic behavior with a resistivity plateau at temperatures lower than 10 K. In this paper, we study the electronic structure of TaTe$_4$ using a combination of high-resolution angle-resolved photoemission spectroscopy and density functional calculations. Our results reveal the existence of the long-sought metallic states. These states exhibit mixed dimensionality, while some of them might have potential topological properties.",2305.00053v1 2023-05-15,Magnetic order and electronic transport properties in the Mn$_3$Al compound: the role of the structural state,"Electronic transport and magnetic properties of bulk and rapid melt quenched samples of the Mn$_3$Al Heusler alloy were studied. A correlation between the magnetic and structural states was established. For a cast sample, there is no ferromagnetic moment, and the behavior of the magnetic susceptibility (break at low temperatures and the Curie-Weiss law with high values of the paramagnetic Curie temperature) indicates a frustrated antiferromagnetic state. At the same time, for a rapid melt quenched sample, a ferrimagnetic state is observed with a moment close to compensation. The results of measurements of the electrical resistivity and the Hall effect evidence as well in favor of the implementation of these magnetic states.",2305.08646v1 2023-06-01,Native defect association in beta-Ga2O3 enables room-temperature p-type conductivity,"The room temperature hole conductivity of the ultra wide bandgap semiconductor beta Ga2O3 is a pre-requisite for developing the next-generation electronic and optoelectronic devices based on this oxide. In this work, high-quality p-type beta-Ga2O3 thin films grown on r-plane sapphire substrate by metalorganic chemical vapor deposition (MOCVD) exhibit Rho = 50000Ohm.cm resistivity at room temperature. A low activation energy of conductivity as Ea2=170 meV was determined, associated to the oxygen - gallium native acceptor defect complex. Further, taking advantage of cation (Zn) doping, the conductivity of Ga2O3:Zn film was remarkably increased by three orders of magnitude, showing a long-time stable room-temperature hole conductivity with the conductivity activation energy of around 86 meV.",2306.01115v1 2023-06-07,Phase formation in hole- and electron-doped rare-earth nickelate single crystals,"The recent discovery of superconductivity in hole-doped infinite-layer nickelates has triggered a great interest in the synthesis of novel nickelate phases, which have primarily been examined in thin film samples. Here, we report the high-pressure optical floating zone (OFZ) growth of various perovskite and perovskite-derived rare-earth nickelate single-crystals, and investigate the effects of hole-, electron-, and self-doping. For hole-doping with Ca and Sr, we observe phase separations during the growth process when a substitution level of 8% is exceeded. A similar trend emerges for electron-doping with Ce and Zr. Employing lower doping levels allows us to grow sizeable crystals in the perovskite phase, which exhibit significantly different electronic and magnetic properties than the undoped parent compounds, such as a decreased resistivity and a suppressed magnetic response. Our insights into the doping-dependent phase formation and the resulting properties of the synthesized crystals reveal limitations and opportunities for the exploration and manipulation of electronic states in rare-earth nickelates.",2306.04157v1 2023-07-21,Superexchange Interaction in Insulating EuZn$_{2}$P$_{2}$,"We report magnetic and transport properties of single-crystalline EuZn$_{2}$P$_{2}$, which has trigonal CaAl$_2$Si$_2$-type crystal structure and orders antiferromagnetically at $\approx$23~K. Easy $ab$-plane magneto-crystalline anisotropy was confirmed from the magnetization isotherms, measured with a magnetic field applied along different crystallographic directions ($ab$-plane and $c$-axis). Positive Curie-Weiss temperature indicates dominating ferromagnetic correlations. Electrical resistivity displays insulating behavior with a band-gap of $\approx\,$0.177~eV, which decreases to $\approx\,$0.13~eV upon application of a high magnetic field. We explained the intriguing presence of magnetic interactions in an intermetallic insulator by the mechanism of extended superexchange, with phosphorus as an anion mediator, which is further supported by our analysis of the charge and spin density distributions. We constructed the effective Heisenberg model, with exchange parameters derived from the \textit{ab initio} DFT calculations, and employed it in Monte-Carlo simulations, which correctly reproduced the experimental value of N\'eel temperature.",2307.11924v1 2023-08-04,Learning to Shape by Grinding: Cutting-surface-aware Model-based Reinforcement Learning,"Object shaping by grinding is a crucial industrial process in which a rotating grinding belt removes material. Object-shape transition models are essential to achieving automation by robots; however, learning such a complex model that depends on process conditions is challenging because it requires a significant amount of data, and the irreversible nature of the removal process makes data collection expensive. This paper proposes a cutting-surface-aware Model-Based Reinforcement Learning (MBRL) method for robotic grinding. Our method employs a cutting-surface-aware model as the object's shape transition model, which in turn is composed of a geometric cutting model and a cutting-surface-deviation model, based on the assumption that the robot action can specify the cutting surface made by the tool. Furthermore, according to the grinding resistance theory, the cutting-surface-deviation model does not require raw shape information, making the model's dimensions smaller and easier to learn than a naive shape transition model directly mapping the shapes. Through evaluation and comparison by simulation and real robot experiments, we confirm that our MBRL method can achieve high data efficiency for learning object shaping by grinding and also provide generalization capability for initial and target shapes that differ from the training data.",2308.02150v1 2023-08-16,Growth of millimeter-sized high-quality CuFeSe$_2$ single crystals by the molten salt method and study of their semiconducting behavior,"An eutectic AlCl$_3$/KCl molten salt method in a horizontal configuration was employed to grow millimeter-sized and composition homogeneous CuFeSe$_2$ single crystals due to the continuous growth process in a temperature gradient induced solution convection. The typical as-grown CuFeSe$_2$ single crystals in cubic forms are nearly 1.6$\times$1.2$\times$1.0 mm3 in size. The chemical composition and homogeneity of the crystals was examined by both inductively coupled plasma atomic emission spectroscopy and energy dispersive spectrometer with Cu:Fe:Se = 0.96:1.00:1.99 consistent with the stoichiometric composition of CuFeSe$_2$. The magnetic measurements suggest a ferrimagnetic or weak ferromagnetic transition below T$_C$ = 146 K and the resistivity reveals a semiconducting behavior and an abrupt increase below T$_C$.",2308.08223v1 2023-08-25,WSTac: Interactive Surface Perception based on Whisker-Inspired and Self-Illuminated Vision-Based Tactile Sensor,"Modern Visual-Based Tactile Sensors (VBTSs) use cost-effective cameras to track elastomer deformation, but struggle with ambient light interference. Solutions typically involve using internal LEDs and blocking external light, thus adding complexity. Creating a VBTS resistant to ambient light with just a camera and an elastomer remains a challenge. In this work, we introduce WStac, a self-illuminating VBTS comprising a mechanoluminescence (ML) whisker elastomer, camera, and 3D printed parts. The ML whisker elastomer, inspired by the touch sensitivity of vibrissae, offers both light isolation and high ML intensity under stress, thereby removing the necessity for additional LED modules. With the incorporation of machine learning, the sensor effectively utilizes the dynamic contact variations of 25 whiskers to successfully perform tasks like speed regression, directional identification, and texture classification. Videos are available at: https://sites.google.com/view/wstac/.",2308.13241v1 2023-09-03,Validation of the Wiedemann-Franz Law in solid and molten tungsten above 2000 K through thermal conductivity measurements via steady state temperature differential radiometry,"We measure the thermal conductivity of solid and molten tungsten using Steady State Temperature Differential Radiometry. We demonstrate that the thermal conductivity can be well described by application of Wiedemann-Franz Law to electrical resistivity data, thus suggesting the validity of Wiedemann-Franz Law to capture the electronic thermal conductivity of metals in their molten phase. We further support this conclusion using ab initio molecular dynamics simulations with a machine-learned potential. Our results show that at these high temperatures, the vibrational contribution to thermal conductivity is negligible compared to the electronic component.",2309.01062v1 2023-10-05,Demonstration of a monocrystalline GaAs-$β$-Ga$_2$O$_3$ p-n heterojunction,"In this work, we report the fabrication and characterizations of a monocrystalline GaAs/$\beta$-Ga$_2$O$_3$ p-n heterojunction by employing semiconductor grafting technology. The heterojunction was created by lifting off and transfer printing a p-type GaAs single crystal nanomembrane to an Al$_2$O$_3$-coated n-type$\beta$-Ga$_2$O$_3$ epitaxial substrate. The resultant heterojunction diodes exhibit remarkable performance metrics, including an ideality factor of 1.23, a high rectification ratio of 8.04E9 at +/- 4V, and a turn on voltage of 2.35 V. Furthermore, at +5 V, the diode displays a large current density of 2500 A/cm$^2$ along with a low ON resistance of 2 m$\Omega\cdot$cm$^2$.",2310.03886v1 2023-11-03,Effects of Cr content on ion-irradiation hardening of FeCrAl ODS ferritic steels with 9 wt\% Al,"FeCrAl ODS steels for accident tolerant fuel claddings are designed to bear high-Cr and Al for enhancing oxidation resistance. In this study, we investigated the effects of Cr content on ion-irradiation hardening of three ODS ferritic steels with different Cr contents added with 9 wt\% Al, Fe12Cr9Al (SP12), Fe15Cr9Al (SP13), and Fe18Cr9Al (SP14). The specimens were irradiated with 6.4MeV Fe\textsuperscript{3+} at 300 \textdegree C to nominal 3 dpa. The irradiation hardening was measured by nanoindentation method, and the Nix-Gao plots were used to evaluate the bulk-equivalent hardness. The results showed that the irradiation hardening decreased with increasing Cr content. The reason is due to the growth of dislocation loops hindered by solute Cr atoms. TEM observations showed both $\langle 100\rangle$ and $1/2\langle 111\rangle$ dislocation loops existed in the irradiated area. The irradiation hardening was estimated by dispersed barrier hardening (DBH) model with dislocation loops.",2311.01879v1 2023-11-11,Evidence of Ordering in Cu-Ni Alloys from Experimental Electronic Entropy Measurements,"Phase diagrams exhibiting extended solid-solution and lens-like melting are often reproduced using ideal solutions, where ideal mixing considers a fully random configurational entropy of mixing. In the field of irreversible thermodynamics, experimental measurements of the composition variation of high-temperature electronic transport and molten-state properties suggest however a strong role for short-range atomic ordering in these systems. Herein, measurements of the thermopower and resistivity are reported for Cu-Ni solid-solutions as a function of temperature and composition. The electronic transport properties were interpreted with an irreversible thermodynamic framework, revealing a large electronic contribution to the entropy of mixing. Through appeal to a cluster model for the configurational entropy that uses the electronic contribution to inform the existence of ordered associates, we rationalize such contribution of the electronic entropy with the notion of an ideal entropy of mixing commonly used to model such systems. These results suggest that the short range order (S.R.O.) of the atoms plays a significant role in both the solid and molten states, even when there are no dominant intermetallic compounds in these alloys.",2311.06603v2 2023-11-12,First-principles pressure dependent investigation of the physical properties of KB2H8: a prospective high-TC superconductor,"Using the density functional theory (DFT) based first-principles investigation, the structural, mechanical, hardness, elastic anisotropy, optoelectronic, and thermal properties of cubic KB2H8 have been studied within the uniform pressure range of 0 - 24 GPa. The calculated structural parameters are in good agreement with the previous theoretical work. The compound KB2H8 is found to be structurally and thermodynamically stable in the pressure range from 8 GPa to 24 GPa. Single crystal elastic constants Cij and bulk elastic moduli (B, G and Y) increase systematically with pressure from 8 GPa to 24 GPa. In the stable phase, KB2H8 is moderately elastically anisotropic and ductile in nature. The compound is highly machinable and fracture resistant. The Debye temperature, melting temperature and thermal conductivity increases with pressure. The results of electronic band structure calculations and optical parameters at different pressures are consistent with each other. The compound is optically isotropic. The compound KB2H8 has potential to be used as a very efficient solar energy reflector. The electronic energy density of states at the Fermi level decreases systematically with increasing pressure. The same trend is found for the repulsive Coulomb pseudopotential. Possible relevance of the studied properties to superconductivity has also been discussed in this paper.",2311.06709v1 2023-12-08,Gate-controlled neuromorphic functional transition in an electrochemical graphene transistor,"Neuromorphic devices have gained significant attention as potential building blocks for the next generation of computing technologies owing to their ability to emulate the functionalities of biological nervous systems. The essential components in artificial neural network such as synapses and neurons are predominantly implemented by dedicated devices with specific functionalities. In this work, we present a gate-controlled transition of neuromorphic functions between artificial neurons and synapses in monolayer graphene transistors that can be employed as memtransistors or synaptic transistors as required. By harnessing the reliability of reversible electrochemical reactions between C atoms and hydrogen ions, the electric conductivity of graphene transistors can be effectively manipulated, resulting in high on/off resistance ratio, well-defined set/reset voltage, and prolonged retention time. Overall, the on-demand switching of neuromorphic functions in a single graphene transistor provides a promising opportunity to develop adaptive neural networks for the upcoming era of artificial intelligence and machine learning.",2312.04934v2 2023-12-20,Collective dynamics and long-range order in thermal neuristor networks,"In the pursuit of scalable and energy-efficient neuromorphic devices, recent research has unveiled a novel category of spiking oscillators, termed ""thermal neuristors"". These devices function via thermal interactions among neighboring vanadium dioxide resistive memories, emulating biological neuronal behavior. Here, we show that the collective dynamical behavior of networks of these neurons showcases a rich phase structure, tunable by adjusting the thermal coupling and input voltage. Notably, we identify phases exhibiting long-range order that, however, does not arise from criticality, but rather from the time non-local response of the system. In addition, we show that these thermal neuristor arrays achieve high accuracy in image recognition and time series prediction through reservoir computing, without leveraging long-range order. Our findings highlight a crucial aspect of neuromorphic computing with possible implications on the functioning of the brain: criticality may not be necessary for the efficient performance of neuromorphic systems in certain computational tasks.",2312.12899v2 2024-01-30,Momentum Matching for 2D-3D Heterogeneous Ohmic van der Waals Contact,"Construction of ohmic contact is a long-standing challenge encountered by two-dimensional (2D) device fabrication and integration. van der Waals contacts, as a new solution for 2D contact construction, can effectively eliminate issues, such as Fermi-level pining and formation of Schottky barrier. Nevertheless, current research primarily considers energy band alignment, while ignoring the transverse momentum conservation of charge carriers during the quantum tunneling across the van der Waals contacts. In this study, by comparing the IV characteristics and tunneling spectra of graphene-silicon tunneling junctions with various interfacial transverse momentum distribution, we demonstrate the importance of charge carrier momentum in constructing high-performance 2D contact. Further, by conditioning the van der Waals contacts and minimizing the momentum mismatch, we successfully enhanced the quantum tunneling current with more than three orders of magnitude and obtain ohmic-like contact. Our study provide and effective method for the construction of direction 2D-3D contact with low resistance and can potentially benefit the heterogeneous of integration of 2D materials in post-CMOS architectures.",2401.17114v1 2024-02-11,Langmuir-like model of dilute impurities in concentrated solid solutions,"High-entropy alloys have drawn recent interest for their promising mechanical properties and irradiation resistance. Various properties, namely transport properties, are controlled by point defect concentration, which must be known before performing atomistic simulations to compute transport coefficients. In this work, we present a general Langmuir-like model for impurity concentration in an arbitrarily complex solid solution and apply this model to generate expressions for concentrations of vacancies and small interstitial atoms. We then calculate the vacancy concentration as a function of temperature in the equiatomic CoNiCrFeMn and FeAl alloys with modified embedded-atom-method potentials for various chemical orderings, showing there is no clear correlation between vacancy thermodynamics and chemical ordering in the CoNiCrFeMn alloy but clear systematic patterns for FeAl.",2402.07324v1 2024-02-28,Strange metal in the doped Hubbard model via percolation,"Many strongly correlated systems, including high-temperature superconductors such as the cuprates, exhibit strange metallic behavior in certain parameter regimes characterized by anomalous transport properties that are irreconcilable with a Fermi-liquid-like description in terms of quasiparticles. The Hubbard model is a standard theoretical starting point to examine the properties of such systems and also exhibits non-Fermi-liquid behavior in simulations. Here we analytically study the two-dimensional hole-doped Hubbard model, first identifying a percolation transition that occurs in the low-energy sector at critical hole doping $p_c\sim 0.19$. We then use the critical properties near this transition to rewrite the Hubbard Hamiltonian in a way that motivates a large-$N$ model with strange metallic properties. In particular, we show that this model has the linear-in-$T$ resistivity and power-law optical conductivity $\sim |\omega|^{-2/3}$ observed in the strange metal regime of cuprates, suggesting potential relevance for describing this important class of materials.",2402.18626v2 2024-03-25,Facile synthesis of micro-flower NiCo2O4 assembled by nanosheets efficient for electrocatalysis of water,"Effective regulation of the morphology of transition metal spinel structures is crucial for creating efficient and stable bifunctional catalysts for electrocatalysis of water. In this work, micro-flower NiCo2O4 (F-NCO) assembled by nanosheets via a chemical template method for the simultaneous promotion of hydrogen evolution reaction (HER) and oxygen evolution reaction (OER). Electronic microscope analysis revealed that the thickness of the F-NCO catalyst was only 2.7% of that of the NiCo2O4 bulk (B-NCO), and this ultrathin lamellar structure was conducive to further exposure of the active site and improved reaction kinetics. The F-NCO catalyst exhibited superior HER and OER performance (10 = 236 and 310 mV) and robust long-term stability over the B-NCO catalyst in 1.0 M KOH, with a 2.68-fold and 4.16-fold increase in active surface area and a 0.42-fold and 0.61-fold decrease in charge transfer resistance values, respectively. This micro-flower-structured electrode has remarkable electrocatalytic property and long-term durability, providing a novel insight for characterizing cost-effective and high-performance bifunctional electrocatalysts.",2403.17744v1 2024-04-30,Aluminum nuclear demagnetization refrigerator for powerful continuous cooling,"Many laboratories routinely cool samples to 10 mK, but relatively few can cool condensed matter below 1 mK. Easy access to the microkelvin range would propel fields such as quantum sensors and quantum materials. Such temperatures are achieved with adiabatic nuclear demagnetization. Existing nuclear demagnetization refrigerators (NDR) are ""single-shot"", and the recycling time is incompatible with proposed sub-mK experiments. Furthermore, a high cooling power is required to overcome the excess heat load of order nW on NDR pre-cooled by cryogen-free dilution refrigerators. We report the performance of an aluminum NDR designed for powerful cooling when part of a dual stage continuous NDR (CNDR). Its thermal resistance is minimized to maximize the cycling rate of the CNDR and consequently its cooling power. At the same time, its susceptibility to eddy current heating is minimized. A CNDR based on two of the aluminum NDR presented here would have a cooling power of approximately 40 nW at 560 $\mu$K.",2404.19352v1 2024-05-10,Effects of vortex and anti-vortex excitations in underdoped Bi-2223 bulk single crystals,"To gain insights into mechanisms underlying superconducting transition in copper oxide high-transition temperature ($T_c$) superconductors, we studied transport properties of underdoped Bi$_2$Sr$_2$Ca$_2$Cu$_3$O$_{10+\delta}$ (Bi-2223) bulk single crystals. The power exponent $\alpha$ ($V \propto I^{\alpha}$) reached 3 just below $T_c$, and the temperature dependence of in-plane resistivity ($\rho_{ab}$) exhibited typical tailing behavior, consistent with Kosterlitz--Thouless transition characteristics. Thus, with increasing temperature, copper oxide high-$T_c$ superconductors undergo transition to the normal state because of destruction of its phase correlations, although a finite Cooper pair density exists at $T_c$.",2405.06272v1 2024-05-15,Unraveling impacts of polycrystalline microstructures on ionic conductivity of ceramic electrolytes by computational homogenization and machine learning,"The ionic conductivity at the grain boundaries (GBs) in oxide ceramics is typically several orders of magnitude lower than that within the grain interior. This detrimental GB effect is the main bottleneck for designing high-performance ceramic electrolytes intended for use in solid-state Lithium-ion batteries, fuel cells, and electrolyzer cells. The macroscopic ionic conductivity in oxide ceramics is essentially governed by the underlying polycrystalline microstructures where GBs and grain morphology go hand in hand. This provides the possibility to enhance the ion conductivity by microstructure engineering. To this end, a thorough understanding of microstructure-property correlation is highly desirable. In this work, we investigate numerous polycrystalline microstructure samples with varying grain and grain boundary features. Their macroscopic ionic conductivities are numerically evaluated by the finite element homogenization method, whereby the GB resistance is explicitly regarded. The influence of different microstructural features on the effective ionic conductivity is systematically studied. The microstructure-property relationships are revealed. Additionally, a graph neural network-based machine learning model is constructed and trained. It can accurately predict the effective ionic conductivity for a given polycrystalline microstructure. This work provides crucial quantitative guidelines for optimizing the ionic conducting performance of oxide ceramics by tailoring microstructures.",2405.09227v1 2024-05-20,High-Mobility Carriers in Epitaxial IrO2 Films Grown using Hybrid Molecular Beam Epitaxy,"Binary rutile oxides of 5d metals such as IrO2, stand out as a paradox due to limited experimental studies despite the rich predicted quantum phenomena. Here, we investigate the electrical transport properties of IrO2 by engineering epitaxial thin films grown via hybrid molecular beam epitaxy. Our findings reveal phonon-limited carrier transport and thickness-dependent anisotropic in-plane resistance in IrO2 (110) films, the latter suggesting a complex relationship between strain relaxation and orbital hybridization. Magneto-transport measurements reveal a previously unobserved non-linear Hall effect. A two-carrier analysis of this effect shows the presence of minority carriers with mobility exceeding 3000 cm2/Vs at 1.8 K. These results point towards emergent properties in 5d metal oxides that can be controlled using dimensionality and epitaxial strain.",2405.11716v1 2024-05-21,A single crystal study of Kagome metals U$_2$Mn$_3$Ge and U$_2$Fe$_3$Ge,"Single crystals of U$_2$Mn$_3$Ge and and U$_2$Fe$_3$Ge with a Kagome lattice structure were synthesized using a high-temperature self-flux crystal growth method. The physical properties of these crystals were characterized through measurements of resistivity, magnetism, and specific heat. U$_2$Fe$_3$Ge exhibits ferromagnetic ground state and Anomalous Hall Effect, and U$_2$Mn$_3$Ge demonstrates a complex magnetic structure. Both compounds exhibit large Sommerfeld coefficient, indicating coexistence of heavy Fermion behavior with magnetism. Our results suggest that this U$_2$TM$_3$Ge (TM = Mn, Fe, Co) family is a promising platform to investigate the interplay of magnetism, Kondo physics and the Kagome lattice.",2405.12905v1 2007-07-30,Control of the Casimir force by the modification of dielectric properties with light,"The experimental demonstration of the modification of the Casimir force between a gold coated sphere and a single-crystal Si membrane by light pulses is performed. The specially designed and fabricated Si membrane was irradiated with 514 nm laser pulses of 5 ms width in high vacuum leading to a change of the charge-carrier density. The difference in the Casimir force in the presence and in the absence of laser radiation was measured by means of an atomic force microscope as a function of separation at different powers of the absorbed light. The total experimental error of the measured force differences at a separation of 100 nm varies from 10 to 20% in different measurements. The experimental results are compared with theoretical computations using the Lifshitz theory at both zero and laboratory temperatures. The total theoretical error determined mostly by the uncertainty in the concentration of charge carriers when the light is incident is found to be about 14% at separations less than 140 nm. The experimental data are consistent with the Lifshitz theory at laboratory temperature, if the static dielectric permittivity of high-resistivity Si in the absence of light is assumed to be finite. If the dc conductivity of high-resistivity Si in the absence of light is included into the model of dielectric response, the Lifshitz theory at nonzero temperature is shown to be experimentally inconsistent at 95% confidence. The demonstrated phenomenon of the modification of the Casimir force through a change of the charge-carrier density is topical for applications of the Lifshitz theory to real materials in fields ranging from nanotechnology and condensed matter physics to the theory of fundamental interactions.",0707.4390v1 2014-09-03,The influence of the Al stabilizer layer thickness on the normal zone propagation velocity in high current superconductors,"The stability of high-current superconductors is challenging in the design of superconducting magnets. When the stability requirements are fulfilled, the protection against a quench must still be considered. A main factor in the design of quench protection systems is the resistance growth rate in the magnet following a quench. The usual method for determining the resistance growth in impregnated coils is to calculate the longitudinal velocity with which the normal zone propagates in the conductor along the coil windings. Here, we present a 2D numerical model for predicting the normal zone propagation velocity in Al stabilized Rutherford NbTi cables with large cross section. By solving two coupled differential equations under adiabatic conditions, the model takes into account the thermal diffusion and the current redistribution process following a quench. Both the temperature and magnetic field dependencies of the superconductor and the metal cladding materials properties are included. Unlike common normal zone propagation analyses, we study the influence of the thickness of the cladding on the propagation velocity for varying operating current and magnetic field. To assist in the comprehension of the numerical results, we also introduce an analytical formula for the longitudinal normal zone propagation. The analysis distinguishes between low-current and high-current regimes of normal zone propagation, depending on the ratio between the characteristic times of thermal and magnetic diffusion. We show that above a certain thickness, the cladding acts as a heat sink with a limited contribution to the acceleration of the propagation velocity with respect to the cladding geometry. Both numerical and analytical results show good agreement with experimental data.",1409.1186v1 2020-01-10,A barrier/seed system for electroless metallization on complex surfaces using (aminomethylaminoethyl)phenethyltrimethoxysilane self-assembled films,"High frequency signals propagate along the edges of conductors. If the conductors are electroplated, then the seed layer forms at least one edge, so care must be taken to insure the electrical quality of these layers. In this work, we study the initial quality of SAM-based seed layers that are compatible with complex surfaces including through-silicon vias (TSVs), as are used in via-last three-dimensional semiconductor device packaging. The conformal and electrical quality of the seed metal is very important. Also important for a multifunction seed layer is its ability as a barrier layer, which protects the substrate from high temperature diffusion of the deposited metal. Thus, the barrier layer must be robust enough to withstand diffusion, yet thin enough to provide a conformal surface that allows metal seed layer deposition. Standard barrier layer deposition methods such as evaporation or sputtering require either a line of sight from the source or aspect ratios large enough to provide scattering from the background gas within the structure to coat all surfaces. Electrochemical and chemical vapor deposition provide alternatives, but concerns arise about contamination and compatibility with radio frequency or high-speed digital signals. We propose a barrier layer based on an aromatic self-assembled monolayer (SAM) for use in electroless copper seed layer deposition. The viability of the SAM barrier layer is determined by the quality of the deposited copper seed film, judged quantitatively by thin film resistivity and qualitatively by surface adhesion and morphological properties such as cracks and bubbles. Insights to the origins of problems and an optimal scheme are described. Extensions for use as a photolithographic resist layer are suggested. Our SAM approach for TSV applications yields a 'smart' seed layer that can be used with a 'simple,' scalloped, easy to fabricate, via hole.",2001.03295v1 2022-04-04,Exceptional fracture toughness of CrCoNi-based medium- and high-entropy alloys close to liquid helium temperatures,"Medium- and high-entropy alloys based on the CrCoNi-system have been shown to display outstanding strength, tensile ductility and fracture toughness (damage-tolerance properties), especially at cryogenic temperatures. Here we examine the JIc and (back-calculated) KJIc fracture toughness values of the face-centered cubic, equiatomic CrCoNi and CrMnFeCoNi alloys at 20 K. At flow stress values of ~1.5 GPa, crack-initiation KJIc toughnesses were found to be exceptionally high, respectively 235 and 415 MPa(square-root)m for CrMnFeCoNi and CrCoNi, with the latter displaying a crack-growth toughness Kss exceeding 540 MPa(square-root)m after 2.25 mm of stable cracking, which to our knowledge is the highest such value ever reported. Characterization of the crack-tip regions in CrCoNi by scanning electron and transmission electron microscopy reveal deformation structures at 20 K that are quite distinct from those at higher temperatures and involve heterogeneous nucleation, but restricted growth, of stacking faults and fine nano-twins, together with transformation to the hexagonal closed-packed phase. The coherent interfaces of these features can promote both the arrest and transmission of dislocations to generate respectively strength and ductility which strongly contributes to sustained strain hardening. Indeed, we believe that these nominally single-phase, concentrated solid-solution alloys develop their fracture resistance through a progressive synergy of deformation mechanisms, including dislocation glide, stacking-fault formation, nano-twinning and eventually in situ phase transformation, all of which serve to extend continuous strain hardening which simultaneously elevates strength and ductility (by delaying plastic instability), leading to truly exceptional resistance to fracture.",2204.01635v1 2023-10-16,Electronic Transport and Fermi Surface Topology of Zintl phase Dirac Semimetal SrZn2Ge2,"We report a comprehensive study on the electronic transport properties of SrZn$_2$Ge$_2$ single crystals. The in-plane electrical resistivity of the compound exhibits linear temperature dependence for 80 K < T < 300 K, and T^2 dependence below 40 K, consistent with the Fermi liquid behavior. Both the transverse and longitudinal magnetoresistance exhibit a crossover at critical field B* from weak-field quadratic-like to high-field unsaturated linear field dependence at low temperatures (T \leq 50 K). Possible sources of linear magnetoresistance are discussed based on the Fermi surface topology, classical and quantum transport models. The Hall resistivity data establish SrZn$_2$Ge$_2$ as a multiband system with contributions from both the electrons and holes. The Hall coefficient is observed to decrease with increasing temperature and magnetic field, changing its sign from positive to negative. The negative Hall coefficient observed at low temperatures in high fields and at high temperatures over the entire field range suggests that the highly mobile electron charge carriers dominate the electronic transport. Our first-principles calculations show that nontrivial topological surface states exist in SrZn$_2$Ge$_2$ within the bulk gap along the {\Gamma}-M path. Notably, these surface states extend from the valence to conduction band with their number varying based on the Sr and Ge termination plane. The Fermi surface of the compound exhibits a distinct tetragonal petal-like structure, with one open and several closed surfaces. Overall, these findings offer crucial insights into the mechanisms underlying the electronic transport of the compound.",2310.10621v2 2023-06-24,High Strength Refractory AlHfNbTiV B2 High Entropy Alloys with High Fracture Strains,"We demonstrate the development of a series of refractory high-entropy alloys containing aluminum AlRHEAs in the ordered BCC-B2 phase by varying the aluminum content within 10 to 25 atomic percent, with the goal of high strength and good ductility synergy. The AlRHEAs obtained are found to show promising potential for high-temperature applications. The incorporation of Al lowers the density and promotes the long-range atomic ordering, which in turn stabilizes the B2 formation, and strengthens the material but usually deteriorates ductility. Several B2 AlRHEAs that contain a combination of Ti, Hf, Nb, and V with moderate to high Poisson ratios are investigated for high strength and ductility. Furthermore, through statistical analysis, we identify a valley around the valence electron concentration VEC of 6 where low ductility is prominently observed. Machine-learning models are employed to screen the vast compositional space of AlRHEA alloys to predict B2 formation and toughness indicated by the yield strength and fracture strain. High prediction accuracies are achieved. As the Al content decreases, the B2 atomic ordering decreases, compression yield strengths decrease from 1500 MPa to 1200 MPa, and compression fracture strains increase from 0.06 to over 0.5. Notably, Al10Hf20Nb22Ti33V15 retains a compression yield strength exceeding 800 MPa up to 700 C, tensile yield strength of 1100 MPa, and fracture strain of 0.083. Our findings on enhancing ductility in pure B2 alloys pave the way for further research on Al-RHEA superalloys, striving to achieve high strength and ductility, reduced density, and improved oxidation resistance.",2306.14057v2 1998-04-04,Ohmic Decay of Magnetic Fields due to non-spherical accretion in the Crusts of Neutron Stars,"We consider magnetic field evolution of neutron stars during polar-cap accretion. The size of the polar cap increases as the field decays, and is set by the last open field line before the accretion disk. Below the polar cap we find the temperature to be so high that electron-phonon scattering dominates the resistivity. Outside the polar cap region, the temperature is such the resistivity is dominated by temperature independent impurity scattering which can be a few orders of magnitude larger than the electron- phonon resistivity. The time-scale for field decay is therefore initially given by impurity scattering dominated resistivity. When the field strength has been reduced to $\sim 10^8 gauss$ the accretion is spherical and the time scale for field decay is given by the smaller electron-phonon scattering resistivity. The field strength is now reduced rapidly compared to before and this could be a reason for there being no pulsars known with field strengths below $10^8 gauss$. We also investigate the evolution of multipoles at the neutron star surface. We find that contribution from higher-order multipoles are at most 30% to that of the dipole mode.",9804047v1 2000-01-10,The Effect of Resistivity on the Nonlinear Stage of the Magnetorotational Instability in Accretion Disks,"We present three-dimensional magnetohydrodynamic simulations of the nonlinear evolution of the magnetorotational instability (MRI) with a non-zero Ohmic resistivity. The properties of the saturated state depend on the initial magnetic field configuration. In simulations with an initial uniform vertical field, the MRI is able to support angular momentum transport even for large resistivities through the quasi-periodic generation of axisymmetric radial channel solutions rather than through the maintenance of anisotropic turbulence. Simulations with zero net flux show that the angular momentum transport and the amplitude of magnetic energy after saturation are significantly reduced by finite resistivity, even at levels where the linear modes are only slightly affected. This occurs at magnetic Reynolds numbers expected in low, cool states of dwarf novae, these results suggest that finite resistivity may account for the low and high angular momentum transport rates inferred for these systems.",0001164v1 1998-10-15,The Quantized Hall Insulator: A New Insulator in Two-Dimensions,"Quite generally, an insulator is theoretically defined by a vanishing conductivity tensor at the absolute zero of temperature. In classical insulators, such as band insulators, vanishing conductivities lead to diverging resistivities. In other insulators, in particular when a high magnetic field (B) is added, it is possible that while the magneto-resistance diverges, the Hall resistance remains finite, which is known as a Hall insulator. In this letter we demonstrate experimentally the existence of another, more exotic, insulator. This insulator, which terminates the quantum Hall effect series in a two-dimensional electron system, is characterized by a Hall resistance which is approximately quantized in the quantum unit of resistance h/e^2. This insulator is termed a quantized Hall insulator. In addition we show that for the same sample, the insulating state preceding the QHE series, at low-B, is of the HI kind.",9810172v1 1999-03-05,Comment on ``Evidence for Anisotropic State of Two-Dimensional Electrons in High Landau Levels'',"In a recent letter M. Lilly et al [PRL 82, 394 (1999)] have shown that a highly anisotropic state can arise in certain two dimensional electron systems. In the large square samples studied, resistances measured in the two perpendicular directions are found to have a ratio that may be 60 or larger at low temperature and at certain magnetic fields. In Hall bar measurements, the anisotropy ratio is found to be much smaller (roughly 5). In this comment we resolve this discrepancy by noting that the anisotropy of the underlying sheet resistivities is correctly represented by Hall bar resistance measurements but shows up exponentially enhanced in resistance measurements on square samples due to simple geometric effects. We note, however, that the origin of this underlying resistivity anisotropy remains unknown, and is not addressed here.",9903086v3 1999-12-01,Fractional-flux Little-Parks resistance oscillations in disordered superconducting Au$_{0.7}$In$_{0.3}$ cylinders,"Resistance of disordered superconducting Au$_{0.7}$In$_{0.3}$ cylindrical films was measured as a function of applied magnetic field. In the high-temperature part of the superconducting transition regime, the resistance oscillated with a period of $h/2e$ in the unit of the enclosed magnetic flux. However, at lower temperatures, the resistance peaks split. We argue that this splitting is due to the emergence of an oscillation with a period of $h/4e$, half of the flux quantum for paired electrons. The possible physical origin of the $h/4e$ resistance oscillation is discussed in the context of new minima in the free energy of a disordered superconducting cylinder.",9912003v3 2000-04-05,Linear response conductance and magneto-resistance of ferromagnetic single-electron transistors,"The current through ferromagnetic single-electron transistors (SET's) is considered. Using path integrals the linear response conductance is formulated as a function of the tunnel conductance vs. quantum conductance and the temperature vs. Coulomb charging energy. The magneto-resistance of ferromagnet-normal metal-ferromagnet (F-N-F) SET's is almost independent of the Coulomb charging energy and is only reduced when the transport dwell time is longer than the spin-flip relaxation time. In all-ferromagnetic (F-F-F) SET's with negligible spin-flip relaxation time the magneto-resistance is calculated analytically at high temperatures and numerically at low temperatures. The F-F-F magneto-resistance is enhanced by higher order tunneling processes at low temperatures in the 'off' state when the induced charges vanishes. In contrast, in the 'on' state near resonance the magneto-resistance ratio is a non-monotonic function of the inverse temperature.",0004082v3 2001-09-10,Transport properties of MgB2,"In this paper we present the resistivity, the Seebeck effect, and the thermal conductivity measurements on a MgB2 sintered sample. Such transport properties highlight the role of the junctions between the grains to a different extent. In particular, the temperature dependence of resistivity may be explained with the assumption that grain boundaries have a resistance, independent of temperature, in series with the resistance of grains. Also the behaviour of the Seebeck effect, as long as the scattering at the grain boundaries is elastic, is not affected at all by granularity. Thus, the thermopower can be a useful tool to provide information on the electronic structure. On the other hand, the grain boundary resistance affects the thermal conductivity strongly, masking the superconducting transition completely.",0109174v2 2003-10-22,Unconventional superconductivity and normal state properties of epsilon-iron at high pressure,"Following the discovery of superconductivity in epsilon-iron, subsequent experiments hinted at non-Fermi liquid behaviour of the normal phase and sensitive dependence of the superconducting state on disorder, both signatures of unconventional pairing. We report further resistive measurements under pressure of samples of iron from multiple sources. The normal state resistivity of epsilon-iron varied as rho_0+AT^{5/3} at low temperature over the entire superconducting pressure domain. The superconductivity could be destroyed by mechanical work, and was restored by annealing, demonstrating sensitivity to the residual resistivity rho_0. There is a strong correlation between the rho_0 and A coefficients and the superconducting critical temperature T_c. Within the partial resistive transition there was a significant current dependence, with V(I)=a(I-I_0)+bI^2, with a >> b, possibly indicating flux-flow resistivity, even in the absence of an externally applied magnetic field.",0310519v1 2003-12-10,Phase slips in superconducting films with constrictions,"A system of two coplanar superconducting films seamlessly connected by a bridge is studied. We observe two distinct resistive transitions as the temperature is reduced. The first one, occurring in the films, shows some properties of the Berezinskii-Kosterlitz-Thouless (BKT) transition. The second apparent transition (which is in fact a crossover) is related to freezing out of thermally activated phase slips (TAPS) localized on the bridge. We also propose a powerful indirect experimental method allowing an extraction of the sample's zero-bias resistance from high-current-bias measurements. Using direct and indirect measurements, we determined the resistance $R(T)$ of the bridges within a range of {\em eleven orders of magnitude}. Over such broad range, the resistance follows a simple relation $R(T)=R_N \text{exp} [-(c/t)(1-t)^{3/2}]$, where $c=\Delta F(0) / kT_c$ is the normalized free energy of a phase slip at zero temperature, $t=T/T_c$ is normalized temperature, and $R_N$ is the normal resistance of the bridge.",0312268v2 2004-10-04,"The ""normal"" state of superconducting cuprates might really be normal after all","High magnetic field studies of cuprate superconductors revealed a non-BCS temperature dependence of the upper critical field $H_{c2}(T)$ determined resistively by several groups. These determinations caused some doubts on the grounds of both the contrasting effect of the magnetic field on the in-plane and out-of-plane resistances reported for large Bi2212 sample and the large Nernst signal \emph{well above} $T_{c}$. Here we present both $\rho_{ab}(B)$ and $\rho_{c}(B)$ of tiny Bi2212 crystals in magnetic fields up to 50 Tesla. None of our measurements revealed a situation when on the field increase $\rho_c$ reaches its maximum while $\rho_{ab}$ remains very small if not zero. The resistive %upper critical fields estimated from the in-plane and out-of-plane $H_{c2}(T)$ estimated from $\rho_{ab}(B)$ and $\rho_{c}(B)$ are approximately the same. Our results support any theory of cuprates that describes the state above the resistive phase transition as perfectly normal with a zero off-diagonal order parameter. In particular, the anomalous Nernst effect above the resistive phase transition in high-$T_{c}$ cuprates can be described quantitatively as a normal state phenomenon in a model with itinerant and localised fermions and/or charged bosons.",0410075v1 2008-04-03,Pressure-temperature Phase Diagram of Polycrystalline UCoGe Studied by Resistivity Measurement,"Recently, coexistence of ferromagnetism (T_Curie = 2.8K) and superconductivity (T_sc = 0.8K) has been reported in UCoGe, a compound close to a ferromagnetic instability at ambient pressure P. Here we present resistivity measurements under pressure on a UCoGe polycrystal. The phase diagram obtained from resistivity measurements on a polycrystalline sample is found to be qualitatively different to those of all other ferromagnetic superconductors. By applying high pressure, ferromagnetism is suppressed at a rate of 1.4 K/GPa. No indication of ferromagnetic order has been observed above P ~ 1GPa. The resistive superconducting transition is, however, quite stable in temperature and persists up to the highest measured pressure of about 2.4GPa. Superconductivity would therefore appear also in the paramagnetic phase. However, the appearance of superconductivity seems to change at a characteristic pressure P* ~ 0.8GPa. Close to a ferromagnetic instability, the homogeneity of the sample can influence strongly the electronic and magnetic properties and therefore bulk phase transitions may differ from the determination by resistivity measurements.",0804.0500v1 2008-08-18,"Upper critical field, anisotropy, and superconducting properties of Ba$_{1-x}$K$_x$Fe$_2$As$_2$ single crystals","The temperature dependent resistivity of Ba$_{1-x}$K$_x$Fe$_2$As$_2$ (x = 0.23, 0.25, 0.28 and 0.4) single crystals and the angle dependent resistivity of superconducting Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$ single crystals were measured in magnetic fields up to 9 T. The measurements of temperature dependent resistivity for samples with different doping levels revealed very high upper critical fields which increase with the transition temperature monotonously, and a very low superconducting anisotropy ratio $\Gamma=H_{c2}^{ab}/H_{c2}^c \approx$ 2. By scaling the resistivity in the frame of the anisotropic Ginzburg-Landau theory, the angle dependent resistivity of the Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$ single crystal measured with different magnetic fields at a certain temperature collapsed onto one curve. As the only scaling parameter, the anisotropy $\Gamma$ was determined alternatively for each temperature and was found to be between two and three.",0808.2392v3 2009-04-28,Complete pressure dependent phase diagrams for SrFe2As2 and BaFe2As2,"The temperature dependent electrical resistivity of single crystalline SrFe2As2 and BaFe2As2 has been measured in a liquid medium, modified Bridgman anvil cell for pressures in excess of 75 kbar. These data allow for the determination of the pressure dependence of the higher temperature, structural / antiferromagnetic phase transitions as well as the lower temperature superconducting phase transition. For both compounds the ambient pressure, higher temperature structural / antiferromagnetic phase transition can be fully suppressed with a dome-like region of zero resistivity found to be centered about its critical pressure. Indeed, qualitatively, the temperature dependence of the resistivity curves closest to the critical pressures are the closest to linear, consistent with possible quantum criticality. For pressures significantly higher than the critical pressure the zero resistivity state is suppressed and the low temperature resistivity curves asymptotically approach a universal, low temperature manifold. These results are consistent with the hypothesis that correlations / fluctuations associated with the ambient-pressure, high-temperature, tetragonal phase have to be brought to low enough temperature to allow superconductivity, but if too fully suppressed can lead to the loss of the superconducting state.",0904.4488v1 2011-01-17,The magnetoresistance and Hall effect in CeFeAsO: a high magnetic field study,"The longitudinal electrical resistivity and the transverse Hall resistivity of CeFeAsO are simultaneously measured up to a magnetic field of 45T using the facilities of pulsed magnetic field at Los Alamos. Distinct behaviour is observed in both the magnetoresistance Rxx({\mu}0H) and the Hall resistance Rxy({\mu}0H) while crossing the structural phase transition at Ts \approx 150K. At temperatures above Ts, little magnetoresistance is observed and the Hall resistivity follows linear field dependence. Upon cooling down the system below Ts, large magnetoresistance develops and the Hall resistivity deviates from the linear field dependence. Furthermore, we found that the transition at Ts is extremely robust against the external magnetic field. We argue that the magnetic state in CeFeAsO is unlikely a conventional type of spin-density-wave (SDW).",1101.3170v1 2013-07-23,"Nonlocal resistance and its fluctuations in microstructures of band-inverted HgTe/(Hg,Cd)Te quantum wells","We investigate experimentally transport in gated microsctructures containing a band-inverted HgTe/Hg_{0.3}Cd_{0.7}Te quantum well. Measurements of nonlocal resistances using many contacts prove that in the depletion regime the current is carried by the edge channels, as expected for a two-dimensional topological insulator. However, high and non-quantized values of channel resistances show that the topological protection length (i.e. the distance on which the carriers in helical edge channels propagate without backscattering) is much shorter than the channel length, which is ~100 micrometers. The weak temperature dependence of the resistance and the presence of temperature dependent reproducible quasi-periodic resistance fluctuations can be qualitatively explained by the presence of charge puddles in the well, to which the electrons from the edge channels are tunnel-coupled.",1307.6115v3 2013-08-01,Resistive Threshold Logic,"We report a resistance based threshold logic family useful for mimicking brain like large variable logic functions in VLSI. A universal Boolean logic cell based on an analog resistive divider and threshold logic circuit is presented. The resistive divider is implemented using memristors and provides output voltage as a summation of weighted product of input voltages. The output of resistive divider is converted into a binary value by a threshold operation implemented by CMOS inverter and/or Opamp. An universal cell structure is presented to decrease the overall implementation complexity and number of components. When the number of input variables become very high, the proposed cell offers advantages of smaller area and design simplicity in comparison with CMOS based logic circuits.",1308.0090v1 2014-02-03,"The Effect of Magnetic Fields, Temperature and Current on the Resistivity of Bi-2223 High Temperature Superconductors","The electrical resistivity of polycrystalline Bi2Sr2Ca2Cu3O10-x (Bi-2223) was measured vs. applied magnetic fields up to 0.45 T, applied currents up to 1 A, and temperature from liquid nitrogen temperature (LN2) to room temperature. In the lowest temperature region, the only truly zero resistivity was observed when the magnetic field was zero; otherwise, a quadratic dependence on the magnetic field occurred. Hysteresis was noted at the higher currents. Current vs. voltage curves in this region revealed a non-ohmic resistivity. In the transition region to the mixed state, indications of negative resistivity and suggestions of a phase change were observed. Arrhenius plots yielded activation energies of around 0.05 eV/molecule. In the mixed state region up to the transition temperature of ~110K, analysis implied that 4 superconducting quantum states exist and that they are cooperatively filled by the superconducting charge carriers. The occupation of the superconducting quantum states is negatively affected by the applied magnetic field and by the applied current. No effect on the polarity or direction of the magnetic field with respect to the direction of the current was observed.",1402.0436v1 2014-10-06,Low Resistance Metal Contacts to MoS2 Devices with Nickel-Etched-Graphene Electrodes,"We report an approach to achieve low-resistance contacts to MoS2 transistors with the intrinsic performance of the MoS2 channel preserved. Through a dry transfer technique and a metal-catalyzed graphene treatment process, nickel-etched-graphene electrodes were fabricated on MoS2 that yield contact resistance as low as 200 ohm-um. The substantial contact enhancement (~2 orders of magnitude) as compared to pure nickel electrodes, is attributed to the much smaller work function of nickel-graphene electrodes, together with the fact that presence of zigzag edges in the treated graphene surface enhances tunneling between nickel and graphene. To this end, the successful fabrication of a clean graphene-MoS2 interface and a low resistance nickel-graphene interface is critical for the experimentally measured low contact resistance. The potential of using graphene as an electrode interlayer demonstrated in this work paves the way towards achieving high performance next-generation transistors.",1410.1328v2 2017-06-14,Kinetic theory of transport for inhomogeneous electron fluids,"The interplay between electronic interactions and disorder is neglected in the conventional Boltzmann theory of transport, yet can play an essential role in determining the resistivity of unconventional metals. When quasiparticles are long-lived, one can account for these intertwined effects by solving spatially inhomogeneous Boltzmann equations. Assuming smooth disorder and neglecting umklapp scattering, we solve these inhomogeneous kinetic equations and compute the electrical resistivity across the ballistic-to-hydrodynamic transition. An important consequence of electron-electron interactions is the modification of the momentum relaxation time; this effect is ignored in the conventional theory. We characterize precisely when interactions enhance the momentum scattering rate, and when they decrease it. Our approach unifies existing semiclassical theories of transport and reveals novel transport mechanisms. In particular, we explain how the resistivity can be proportional to the rate of momentum-conserving collisions. We compare this result with existing transport mysteries, including the disorder-independent $T^2$ resistivity of many Fermi liquids, and the linear-in-$T$ ""Planckian-limited"" resistivity of many strange metals.",1706.04621v3 2017-10-11,Zero-field quantum anomalous Hall metrology as a step towards a universal quantum standard unit system,"In the quantum anomalous Hall effect, the edge states of a ferromagnetically doped topological insulator exhibit quantized Hall resistance and dissipationless transport at zero magnetic field. Up to now, however, the resistance was experimentally assessed with standard transport measurement techniques which are difficult to trace to the von-Klitzing constant R$_K$ with high precision. Here, we present a metrologically comprehensive measurement, including a full uncertainty budget, of the resistance quantization of V-doped (Bi,Sb)$_2$Te$_3$ devices without external magnetic field. We established as a new upper limit for a potential deviation of the quantized anomalous Hall resistance from RK a value of 0.26 +- 0.22 ppm, the smallest and most precise value reported to date. This provides another major step towards realization of the zero-field quantum resistance standard which in combination with Josephson effect will provide the universal quantum units standard in the future.",1710.04090v1 2019-09-20,Phenomenology of anomalous transport in disordered one-dimensional systems,"We study anomalous transport arising in disordered one-dimensional spin chains, specifically focusing on the subdiffusive transport typically found in a phase preceding the many-body localization transition. Different types of transport can be distinguished by the scaling of the average resistance with the system's length. We address the following question: what is the distribution of resistance over different disorder realizations, and how does it differ between transport types? In particular, an often evoked so-called Griffiths picture, that aims to explain slow transport as being due to rare regions of high disorder, would predict that the diverging resistivity is due to fat power-law tails in the resistance distribution. Studying many-particle systems with and without interactions we do not find any clear signs of fat tails. The data is compatible with distributions that decay faster than any power law required by the fat tails scenario. Among the distributions compatible with the data, a simple additivity argument suggests a Gaussian distribution for a fractional power of the resistance.",1909.09507v2 2019-06-29,Ultra-Low Surface Resistance via Vacuum Heat Treatment of Superconducting Radiofrequency Cavities,"We report on an effort to improve the performance of superconducting radiofrequency cavities by the use of heat treatment in a temperature range sufficient to dissociate the natural surface oxide. We find that the residual resistance is significantly decreased, and we find an unexpected reduction in the BCS resistance. Together these result in extremely high quality factor values at relatively large accelerating fields Eacc ~20 MV/m: Q0 of 3-4x10^11 at <1.5 K and Q0 ~5x10^10 at 2.0 K. In one cavity, measurements of surface resistance versus temperature showed an extremely small residual resistance of just 0.63+/-0.06 nOhms at 16 MV/m. SIMS measurements confirm that the oxide was significantly dissociated, but they also show the presence of nitrogen after heat treatment. We also present studies of surface oxidation via exposure to air and to water, as well as the effects of very light surface removal via HF rinse. The possibilities for applications and the planned future development are discussed.",1907.00147v1 2012-03-21,Magnetoplasmon resonance in 2D electron system driven into a zero-resistance state,"We report on a remarkably strong, and a rather sharp, photoresistance peak originating from a dimensional magnetoplasmon resonance (MPR) in a high mobility GaAs/AlGaAs quantum well driven by microwave radiation into a zero-resistance state (ZRS). The analysis of the MPR signalreveals a negative background providing experimental evidence for the concept of absolute negative resistance associated with the ZRS. When a system is further subject to a dc field, the maxima of microwave-induced resistance oscillations decay away and a system reveals a state with close-to-zero differential resistance. The MPR peak, on the other hand, remains essentially unchanged, indicating surprisingly robust Ohmic behavior under the MPR conditions.",1203.4781v1 2015-04-21,Radiation-induced resistance oscillations in a 2D hole gas: a demonstration of a universal effect,"We report on a theoretical insight about the microwave-induced resistance oscillations and zero resistance states when dealing with p-type semiconductors and holes instead of electrons. We consider a high-mobility two-dimensional hole gas hosted in a pure Ge/SiGe quantum well. Similarly to electrons we obtain radiation-induce resistance oscillations and zero resistance states. We analytically deduce a universal expression for the irradiated magnetoresistance, explaining the origin of the minima positions and their $1/4$ cycle phase shift. The outcome is that these phenomena are universal and only depend on radiation and cyclotron frequencies. We also study the possibility of having simultaneously two different carriers driven by radiation: light and heavy holes. As a result the calculated magnetoresistance reveals an interference profile due to the different effective masses of the two types of carriers.",1504.05564v2 2019-10-03,Modeling of Electrical Resistivity of Soil Based on Geotechnical Properties,"Determining the relationship between the electrical resistivity of soil and its geotechnical properties is an important engineering problem. This study aims to develop methodology for finding the best model that can be used to predict the electrical resistivity of soil, based on knowing its geotechnical properties. The research develops several linear models, three non-linear models, and three artificial neural network models (ANN). These models are applied to the experimental data set comprises 864 observations and five variables. The results show that there are significant exponential negative relationships between the electrical resistivity of soil and its geotechnical properties. The most accurate prediction values are obtained using the ANN model. The cross-validation analysis confirms the high precision of the selected predictive model. This research is the first rigorous systematic analysis and comparison of difference methodologies in ground electrical resistivity studies. It provides practical guidelines and examples of design, development and testing non-linear relationships in engineering intelligent systems and applications.",1910.01325v1 2019-10-16,$T$-linear resistivity in models with local self-energy,"A theoretical understanding of the enigmatic linear-in-temperature ($T$) resistivity, ubiquitous in strongly correlated metallic systems, has been a long sought-after goal. Furthermore, the slope of this robust $T$-linear resistivity is also observed to stay constant through crossovers between different temperature regimes: a phenomenon we dub ""slope invariance"". Recently, several solvable models with $T$-linear resistivity have been proposed, putting us in an opportune moment to compare their inner workings in various explicit calculations. We consider two strongly correlated models with local self-energies that demonstrate $T$-linearity: a lattice of coupled Sachdev-Ye-Kitaev (SYK) models and the Hubbard model in single-site dynamical mean-field theory (DMFT). We find that the two models achieve $T$-linearity through distinct mechanisms at intermediate temperatures. However, we also find that these mechanisms converge to an identical form at high temperatures. Surprisingly, both models exhibit ""slope invariance"" across the two temperature regimes. We thus not only reveal some of the diversity in the theoretical inner workings that can lead to $T$-linear resistivity, but we also establish that different mechanisms can result in ""slope invarance"".",1910.07530v2 2020-05-28,Contact resistance extraction of graphene FET technologies based on individual device characterization,"Straightforward contact resistance extraction methods based on electrical device characteristics are described and applied here to graphene field-effect transistors from different technologies. The methods are an educated adaptation of extraction procedures originally developed for conventional transistors by exploiting the drift-diffusion-like transport in graphene devices under certain bias conditions. In contrast to other available approaches for contact resistance extraction of graphene transistors, the practical methods used here do not require either the fabrication of dedicated test structures or internal device phenomena characterization. The methodologies are evaluated with simulation-based data and applied to fabricated devices. The extracted values are close to the ones obtained with other more intricate methodologies. Bias-dependent contact and channel resistances studies, bias-dependent high-frequency performance studies and contact engineering studies are enhanced and evaluated by the extracted contact resistance values.",2005.13926v1 2021-10-29,Influence of Device Geometry on Transport Properties of Topological Insulator Microflakes,"In the transport studies of topological insulators, microflakes exfoliated from bulk single crystals are often used because of the convenience in sample preparation and the accessibility to high carrier mobilities. Here, based on finite element analysis, we show that for the non-Hall-bar shaped topological insulator samples, the measured four-point resistances can be substantially modified by the sample geometry, bulk and surface resistivities, and magnetic field. Geometry correction factors must be introduced for accurately converting the four-point resistances to the longitudinal resistivity and Hall resistivity. The magnetic field dependence of inhomogeneous current density distribution can lead to pronounced positive magnetoresistance and nonlinear Hall effect that would not exist in the samples of ideal Hall bar geometry.",2110.15589v1 2022-04-14,DC-coupled resistive silicon detectors for 4-D tracking,"In this work, we introduce a new design concept: the DC-Coupled Resistive Silicon Detectors, based on the LGAD technology. This new approach intends to address a few known features of the first generation of AC-Coupled Resistive Silicon Detectors (RSD). Our simulation exploits a fast hybrid approach based on a combination of two packages, Weightfield2 and LTSpice. It demonstrates that the key features of the RSD design are maintained, yielding excellent timing and spatial resolutions: a few tens of ps and a few microns. In the presentation, we will outline the optimization methodology and the results of the simulation. We will present detailed studies on the effect of changing the ratio between the n+ layer resistivity and the low-resistivity ring and on the achievable temporal and spatial resolution.",2204.07226v1 2022-10-19,"Vector graphics extraction and analysis of electrical resistance data in Nature volume 586, pages 373-377 (2020)","In this paper, I present an analysis of the electrical resistance graphs in Nature volume 586, pages 373-377 (2020), which reported the discovery of room temperature superconductivity in a carbonaceous sulfur hydride and was subsequently retracted on September 26th, 2022. I show that, over a single temperature interval, the electrical resistance data can be decomposed into at least two signals of differing digital precision, thus raising questions concerning the methods used to obtain the published data. Since the raw data-files for the electrical resistance measurements have not been made available, in order to perform this analysis, I have developed a set of python scripts to extract the data-points with high precision from the internal structure of the vector graphics image files. I describe the data extraction method. Example code and the resulting electrical resistance vs temperature data-files are made available in public repositories.",2210.10766v1 2023-06-26,Towards Optimal Effective Resistance Estimation,"We provide new algorithms and conditional hardness for the problem of estimating effective resistances in $n$-node $m$-edge undirected, expander graphs. We provide an $\widetilde{O}(m\epsilon^{-1})$-time algorithm that produces with high probability, an $\widetilde{O}(n\epsilon^{-1})$-bit sketch from which the effective resistance between any pair of nodes can be estimated, to $(1 \pm \epsilon)$-multiplicative accuracy, in $\widetilde{O}(1)$-time. Consequently, we obtain an $\widetilde{O}(m\epsilon^{-1})$-time algorithm for estimating the effective resistance of all edges in such graphs, improving (for sparse graphs) on the previous fastest runtimes of $\widetilde{O}(m\epsilon^{-3/2})$ [Chu et. al. 2018] and $\widetilde{O}(n^2\epsilon^{-1})$ [Jambulapati, Sidford, 2018] for general graphs and $\widetilde{O}(m + n\epsilon^{-2})$ for expanders [Li, Sachdeva 2022]. We complement this result by showing a conditional lower bound that a broad set of algorithms for computing such estimates of the effective resistances between all pairs of nodes require $\widetilde{\Omega}(n^2 \epsilon^{-1/2})$-time, improving upon the previous best such lower bound of $\widetilde{\Omega}(n^2 \epsilon^{-1/13})$ [Musco et. al. 2017]. Further, we leverage the tools underlying these results to obtain improved algorithms and conditional hardness for more general problems of sketching the pseudoinverse of positive semidefinite matrices and estimating functions of their eigenvalues.",2306.14820v1 2023-08-22,Non-Hermitian topological ohmmeter,"Measuring large electrical resistances forms an essential part of common applications such as insulation testing, but suffers from a fundamental problem: the larger the resistance, the less sensitive a canonical ohmmeter is. Here we develop a conceptually different electronic sensor by exploiting the topological properties of non-Hermitian matrices, whose eigenvalues can show an exponential sensitivity to perturbations. The ohmmeter is realized in an multi-terminal, linear electric circuit with a non-Hermitian conductance matrix, where the target resistance plays the role of the perturbation. We inject multiple currents and measure a single voltage in order to directly obtain the value of the resistance. The relative accuracy of the device increases exponentially with the number of terminals, and for large resistances outperforms a standard measurement by over an order of magnitude. Our work paves the way towards leveraging non-Hermitian conductance matrices in high-precision sensing.",2308.11367v1 2019-09-12,Analysis of RF losses and material characterization of samples removed from a Nb3Sn-coated superconducting RF cavity,"Nb3Sn (Tc ~ 18 K and Hsh ~ 400 mT) is a prospective material to replace Nb (Tc ~ 9 K and Hsh ~ 200 mT) in SRF accelerator cavities for significant cost reduction and performance enhancement. Because of its material properties, Nb3Sn is best employed as a thin film (coating) inside an already built RF cavity structure. A particular test cavity noted as C3C4 was a 1.5 GHz single-cell Nb cavity, coated with Nb3Sn using Sn vapor diffusion process at Jefferson Lab. Cold measurements of the coated cavity indicated the superconducting transition temperature of about 18 K. Subsequent RF measurements indicated field-dependent surface resistance both at 4.3 K and 2.0 K. After initial cold measurements, the cavity RF loss distribution was studied with a thermometry mapping system. Loss regions were identified with thermometry and were cut out for material analysis. The presence of significantly thin patchy regions and other carbon-rich defects is associated with strong local field-dependent surface resistance. This paper summarizes RF and thermometry results correlated with material science findings.",1909.05695v1 2020-02-27,A simple approach to bulk bioinspired tough ceramics,"The development of damage-resistant structural materials that can withstand harsh environments is a major issue in materials science and engineering. Bioinspired brick-and-mortar designs have recently demonstrated a range of interesting mechanical properties in proof-of-concept studies. However, reproducibility and scalability issues associated with the actual processing routes have impeded further developments and industrialization of such materials. Here we demonstrate a simple approach based on uniaxial pressing and field assisted sintering of commercially available raw materials to process bioinspired ceramic/ceramic composites of larger thickness than previous approaches, with a sample thickness up to 1 cm. The ceramic composite retains the strength typical of dense alumina ($430~\pm 30MPa$) while keeping the excellent damage resistance demonstrated previously at the millimeter scale with a crack initiation toughness of $6.6MPa.m^{1/2}$ and fracture toughness up to $17.6 MPa.m^{1/2}$. These results validate the potential of these all-ceramic composites, previously demonstrated at lab scale only, and could enable their optimization, scale-up, and industrialization.",2003.11898v1 2021-10-09,Fracture Diodes: Directional asymmetry of fracture toughness,"Toughness describes the ability of a material to resist fracture or crack propagation. It is demonstrated here that fracture toughness of a material can be asymmetric, i.e., the resistance of a medium to a crack propagating from right to left can be significantly different from that to a crack propagating from left to right. Such asymmetry is unknown in natural materials, but we show that it can be built into artificial materials through the proper control of microstructure. This paves the way for control of crack paths and direction, where fracture -- when unavoidable -- can be guided through pre-designed paths to minimize loss of critical components.",2110.04613v1 2022-07-20,Do thermoelectric generator modules degrade due to nickel diffusion,"The paper shows by calculation that the diffusion of nickel even for 50 years does not lead to degradation of thermoelectric generator modules. In the process, we used the theory of composites to calculate the electrical contact resistance, our own diffusion theory of electrical contact resistance, as well as the method for approximating the temperature dependences of thermoelectric material characteristics from the experimental data. When using the above method, it was assumed that the main mechanism of scattering of free charge carriers in a thermoelectric material is their scattering on the deformation potential of acoustic phonons with a free path length independent of energy but inversely proportional to temperature, and the main mechanism of phonon scattering is phonon-phonon scattering with Umklapp, which is not affected by the nickel impurity in the thermoelectric material. Thus, it was believed that the role of nickel is reduced only to a change in the concentration of free charge carriers in the material.",2207.12122v1 2023-03-10,Engineering heat transport across epitaxial lattice-mismatched van der Waals heterointerfaces,"Artificially engineered 2D materials offer unique physical properties for thermal management, surpassing naturally occurring materials. Here, using van der Waals epitaxy, we demonstrate the ability to engineer extremely insulating ultra-thin thermal metamaterials based on crystalline lattice-mismatched Bi2Se3/MoSe2 superlattices and graphene/PdSe2 heterostructures with exceptional thermal resistances (70-202 m^2K/GW) and ultralow cross-plane thermal conductivities (0.01-0.07 Wm^-1K^-1) at room temperature, comparable to those of amorphous materials. Experimental data obtained using frequency-domain thermoreflectance and low-frequency Raman spectroscopy, supported by tight-binding phonon calculations, reveal the impact of lattice mismatch, phonon-interface scattering, size effects, temperature and interface thermal resistance on cross-plane heat dissipation, uncovering different thermal transport regimes and the dominant role of long-wavelength phonons. Our findings provide essential insights into emerging synthesis and thermal characterization methods and valuable guidance for the development of large-area heteroepitaxial van der Waals films of dissimilar materials with tailored thermal transport characteristics.",2303.05808v1 2023-09-25,Integrated bolometric photodetectors based on transparent conductive oxides from near- to mid-infrared wavelengths,"On-chip photodetectors are essential components in optical communications as they convert light into an electrical signal. Photobolometers are type of photodetector that functions through a resistance change caused by electronic temperature fluctuations upon light absorption. They are widely used in the broad wavelength range from UV to MIR and can operate on a wide material platform. In this work, I introduce a novel waveguide-integrated bolometer that operates in a wide wavelength range from NIR to MIR on the standard material platform with the transparent conductive oxides (TCOs) as the active material. This material platform enables the construction of both modulators and photodetectors using the same material, which is fully CMOS compatible and easily integrated with passive on-chip components. The photobolometers proposed here consist of a thin TCO layer placed inside the rib photonic waveguide to enhance light absorption and then heat the electrons in the TCO to temperatures above 1000 K. This rise in electron temperature leads to decreasing electron mobility and consequential electrical resistance change. In consequence, a responsivity exceeding 10 A/W can be attained with a mere few microwatts of optical input power. Calculations suggest that further improvements can be expected with lower doping of the TCO, thus opening new doors in on-chip photodetectors.",2309.14454v1 2023-10-04,Current-driven magnetic resistance in van der Waals spin-filter antiferromagnetic tunnel junctions with MnBi$_2$Te$_4$,"The field of 2D magnetic materials has paved the way for the development of spintronics and nanodevices with new functionalities. Utilizing antiferromagnetic materials, in addition to layered van der Waals (vdW) ferromagnetic materials, has garnered significant interest. In this work, we present a theoretical investigation of the behavior of MnBi$_2$Te$_4$ devices based on the non-equilibrium Green's function method. Our results show that the current-voltage (I-V) characteristics can be influenced significantly by controlling the length of the device and bias voltage and thus allow us to manipulate the tunneling magneto-resistance (TMR) with an external bias voltage. This can be further influenced by the presence of the boron nitride layer which shows significantly enhanced TMR by selectively suppressing specific spin channels for different magnetic configurations. By exploiting this mechanism, the observed TMR value reaches up to 3690\%, which can be attributed to the spin-polarized transmission channel and the projected local density of states. Our findings on the influence of structural and magnetic configurations on the spin-polarized transport properties and TMR ratios give the potential implementation of antiferromagnetic vdW layered materials in ultrathin spintronics.",2310.02830v1 2019-05-04,"Pressure enhanced interplay among lattice, spin and charge in La2FeMnO6 mixed perovskite","Spin crossover plays a central role in the structural instability, net magnetic moment modification, metallization, and even in superconductivity in corresponding materials. Most reports on the pressure-induced spin crossover with a large volume collapse so far focused on compounds with single transition metal. Here we report a comprehensive high-pressure investigation of a mixed Fe-Mn perovskite La2FeMnO6. Under pressure, the strong coupling between Fe and Mn leads to a combined valence/spin transition: Fe3+(S = 5/2) to Fe2+(S = 0) and Mn3+(S = 2) to Mn4+(S = 3/2), with an isostructural phase transition. The spin transitions of both Fe and Mn are offset by ~ 20 GPa of the onset pressure, and the lattice collapse occurs in between. Interestingly, Fe3+ ion shows an abnormal behavior when it reaches a lower valence state (Fe2+) accompanied by a + 0.5 eV energy shift in Fe K-absorption edge at 15 GPa. This process is associated with the charge-spin-orbital state transition from high spin Fe3+ to low spin Fe2+, caused by the significantly enhanced t2g-eg crystal field splitting in the compressed lattice under high pressure. Density Functional Theory calculations confirm the energy preference of the high-pressure state with charge redistribution accompanied by spin state transition of Fe ions. Moreover, La2FeMnO6 maintains semiconductor behaviors even when the pressure reached 144.5 GPa as evidenced by the electrical transport measurements, despite the huge resistivity decreasing 7 orders of magnitude compared with that at ambient pressure. The investigation carried out here demonstrates high flexibility of double perovskites and their good potentials for optimizing the functionality of these materials.",1905.01521v1 2012-03-16,Development and preliminary tests of resistive microdot and microstrip detectors,"In the last few years our group have focused on developing various designs of spark-protected micropattern gaseous detectors featuring resistive electrodes instead of the traditional metallic ones: resistive microstrip counters, resistive GEM, resistive MICROMEGAS. These detectors combine in one design the best features of RPCs (spark-protection) and micropattern detectors (a high position resolution). In this paper we report the progress so far made in developing other types of resistive micropattern detectors: a microdot-microhole detector and a microgap-microstrip detector. The former detector is an optimal electron amplifier for some special designs of dual phase noble liquid TPCs, for example with a CsI photocathode immersed inside the noble liquid. Preliminary tests of such a detector, for the first time built and investigated, are reported in this paper. The latter detector is mainly orientated towards medical imaging applications such as X-ray scanners. However, we believe that after a proper gas optimization, these detectors could also achieve a high time resolution and could thus be used in applications as TOF-PET, detection of charged particles with simultaneous high time and position resolution etc.",1203.3658v2 2022-10-25,Stopping Resistance Drift in Phase Change Memory Cells and Analysis of Charge Transport in Stable Amorphous Ge2Sb2Te5,"We stabilize resistance of melt-quenched amorphous Ge2Sb2Te5 (a-GST) phase change memory (PCM) line cells by substantially accelerating resistance drift and bringing it to a stop within a few minutes with application of high electric field stresses. The acceleration of drift is clearly observable at electric fields > 26 MV/m at all temperatures (85 K - 300 K) and is independent of the current forced through the device, which is a strong function of temperature. The low-field (< 21 MV/m) I-V characteristics of the stabilized cells measured in 85 K - 300 K range fit well to a 2D thermally-activated hopping transport model, yielding hopping distances in the direction of the field and activation energies ranging from 2 nm and 0.2 eV at 85 K to 6 nm and 0.4 eV at 300 K. Hopping transport appears to be better aligned with the field direction at higher temperatures. The high-field current response to voltage is significantly stronger and displays a distinctly different characteristic: the differential resistances at different temperatures extrapolate to a single point (8.9x10-8 ohm.cm), comparable to the resistivity of copper at 60 K, at 65.6 +/- 0.4 MV/m. The physical mechanisms that give rise to the substantial increase in current in the high-field regime also accelerate resistance drift. We constructed field and temperature dependent conduction models based on the experimental results and integrated it with our electro-thermal finite element device simulation framework to analyze reset, set and read operations of PCM devices.",2210.14035v1 2013-07-08,5d transition metal oxide IrO2 as a material for spin current detection,"Devices based on a pure spin current (a flow of spin angular momentum) have been attracting increasing attention as key ingredients for low-dissipation electronics. To integrate such spintronics devices into charge-based technologies, an electric detection of spin current is essential. Inverse spin Hall effect converts a spin current into an electric voltage through spin-orbit coupling. Noble metals such as Pt and Pd, and also Cu-based alloys, owing to the large direct spin Hall effect, have been regarded as potential materials for a spin-current injector. Those materials, however, are not promising as a spin-current detector based on inverse spin Hall effect. Their spin Hall resistivity rho_SH, representing the performance as a detector, is not large enough mainly due to their low charge resistivity. Here we demonstrate that heavy transition metal oxides can overcome such limitations inherent to metal-based spintronics materials. A binary 5d transition metal oxide IrO2, owing to its large resistivity as well as a large spin-orbit coupling associated with 5d character of conduction electrons, was found to show a gigantic rho_SH ~ 38 microohm cm at room temperature, one order of magnitude larger than those of noble metals and Cu-based alloys and even comparable to those of atomic layer thin film of W and Ta.",1307.2121v1 2018-10-31,Challenges in materials and devices for Resistive-Switching-based Neuromorphic Computing,"This tutorial describes challenges and possible avenues for the implementation of the components of a solid-state system, which emulates a biological brain. The tutorial is devoted mostly to a charge-based (i.e. electric controlled) implementation using transition metal oxides materials, which exhibit unique properties that emulate key functionalities needed for this application. In the Introduction, we compare the main differences between a conventional computational machine, based on the Turing-von Neumann paradigm, to a Neuromorphic machine, which tries to emulate important functionalities of a biological brain. We also describe the main electrical properties of biological systems, which would be useful to implement in a charge-based system. In Chapter II, we describe the main components of a possible solid-state implementation. In Chapter III, we describe a variety of Resistive Switching phenomena, which may serve as the functional basis for the implementation of key devices for Neuromorphic computing. In Chapter IV we describe why transition metal oxides, are promising materials for future Neuromorphic machines. Theoretical models describing different resistive switching mechanisms are discussed in Chapter V while existing implementations are described in Chapter VI. Chapter VII presents applications to practical problems. We list in Chapter VIII important basic research challenges and open issues. We discuss issues related to specific implementations, novel materials, devices and phenomena. The development of reliable, fault tolerant, energy efficient devices, their scaling and integration into a Neuromorphic computer may bring us closer to the development of a machine that rivals the brain.",1812.01120v1 2023-01-25,$T-$linear resistivity from magneto-elastic scattering: application to PdCrO$_2$,"An electronic solid with itinerant carriers and localized magnetic moments represents a paradigmatic strongly correlated system. The electrical transport properties associated with the itinerant carriers, as they scatter off these local moments, has been scrutinized across a number of materials. Here we analyze the transport characteristics associated with ultra-clean PdCrO$_2$ -- a quasi two-dimensional material consisting of alternating layers of itinerant Pd-electrons and Mott-insulating CrO$_2$ layers -- which shows a pronounced regime of $T-$linear resistivity over a wide-range of intermediate temperatures. By contrasting these observations to the transport properties in a closely related material PdCoO$_2$, where the CoO$_2$ layers are band-insulators, we can rule out the traditional electron-phonon interactions as being responsible for this interesting regime. We propose a previously ignored electron-magnetoelastic interaction between the Pd-electrons, the Cr local-moments and an out-of-plane phonon as the main scattering mechanism that leads to the significant enhancement of resistivity and a $T-$linear regime in PdCrO$_2$ at temperatures far in excess of the magnetic ordering temperature. We suggest a number of future experiments to confirm this picture in PdCrO$_2$, as well as other layered metallic/Mott-insulating materials.",2301.10776v2 2011-11-14,Nanostructuring of Ba8Ga16Ge30 clathrates,"First thermoelectric properties measurements on bulk nanostructured Ba8Ga16Ge30 clathrate-I are presented. A sol-gel-calcination route was developed for preparing amorphous nanosized precursor oxides. The further reduction of the oxides led to quantitative yield of crystalline nanosized Ba8Ga16Ge30 clathrate-I. TEM investigations show the clathrate nanoparticles retain the size and morphology of the precursor oxides. The clathrate nanoparticles contain mainly thin plates (approx. 300 nm x 300 nm x 50 nm) and a small amount of nanospheres (diameter ~ 10 nm). SAED patterns confirm the clathrate-I structure type for both morphologies. The powders were compacted via Spark Plasma Sintering (SPS) to obtain a bulk nano-structured material. The Seebeck coefficient S, measured on low-density samples (53% of {\delta}x-ray), reaches -145 {\mu}V/k at 375 {\deg}C. The ZT values are quite low (0.02) due to the high resistivity of the sample (two orders of magnitude larger than bulk materials) and the low sample density. The trend of the temperature dependence of S is in agreement with the values obtained from electronic structure calculations and semi-classical Boltzmann transport theory within the constant scattering approximation. The total thermal conductivity (1.61 W/mK), measured on high density samples (93% of {\delta}x-ray), shows a reduction of 20-25% in relation to the bulk materials (2.1 W/mK). A further shaping of the sample for the Seebeck coefficient and electrical conductivity measurements was not possible due to the presence of cracks. An improvement on the design of the pressing tools, loading of the sample and profile of the applied pressure will enhance the mechanical stability of the samples. These investigations are now in progress.",1111.3233v1 2013-02-10,"Synthesis and properties of charge-ordered thallium halide perovskites, CsTl1+0.5Tl3+0.5X3 (X = F, Cl)- theoretical precursors for superconductivity?","Recently CsTlCl3 and CsTlF3 perovskites were theoretically predicted to be potential superconductors if they are optimally doped. The synthesis of these two compounds, together with a complete characterization of the samples are reported. CsTlCl3 is obtained as orange crystals in two different polymorphs: a tetragonal (I4/m) and a cubic (Fm-3m) phase. CsTlF3 is formed as a light brown powder, also as a double cubic perovskite (Fm-3m). In all three CsTlX3 phases Tl1+ and Tl3+ were located in two different crystallographic positions that accommodate their different bond lengths. In CsTlCl3 some Tl vacancies are found in the Tl1+ position. The charge ordering between Tl1+ and Tl3+ was confirmed by x-ray absorption and Raman spectroscopy. The Raman spectroscopy of CsTlCl3 under high pressure (58 GPa) did not indicate any phase transition to a possible single Tl2+ state. However, the highly insulating material becomes less resistive with increasing high pressure, while undergoing a change in the optical properties, from transparent to deeply opaque red, indicative of a decrease of the band gap. The theoretical design and experimental validation of the existence of CsTlF3 and CsTlCl3 cubic perovskites is the necessary first step in confirming the theoretical prediction of superconductivity in these materials.",1302.2353v3 2021-03-28,Radiation-tolerant high-entropy alloys via interstitial-solute-induced chemical heterogeneities,"High-entropy alloys (HEAs) composed of multiple principal elements have been shown to offer improved radiation resistance over their elemental or dilute-solution counterparts. Using NiCoFeCrMn HEA as a model, here we introduce carbon and nitrogen interstitial alloying elements to impart chemical heterogeneities in the form of the local chemical order (LCO) and associated compositional variations. Density functional theory simulations predict chemical short-range order (CSRO) (nearest neighbors and the next couple of atomic shells) surrounding C and N, due to the chemical affinity of C with (Co, Fe) and N with (Cr, Mn). Atomic-resolution chemical mapping of the elemental distribution confirms marked compositional variations well beyond statistical fluctuations. Ni+ irradiation experiments at elevated temperatures demonstrate a remarkable reduction in void swelling by at least one order of magnitude compared to the base HEA without C and N alloying. The underlying mechanism is that the interstitial-solute-induced chemical heterogeneities roughen the lattice as well as the energy landscape, impeding the movements of, and constraining the path lanes for, the normally fast-moving self-interstitials and their clusters. The irradiation-produced interstitials and vacancies therefore recombine more readily, delaying void formation. Our findings thus open a promising avenue towards highly radiation-tolerant alloys.",2103.15134v1 2024-01-21,Hydrostatic pressure effect on structural and transport properties of co-existing layered and disordered rock-salt phase of LixCoO2,"It is widely believed that the origin of a significant cause for the voltage and capacity fading observed in lithium (Li)-ion batteries is related to structural modifications occurring in the cathode material during the Li-ion insertion/de-insertion process. The Li-ion insertion/de-insertion mechanism and the resulting structural changes are known to exert a severe strain on the lattice, and consequently leading to performance degradation. Here, with a view to shed more light on the effect of such strain on the structural properties of the cathode material, we have systematically investigated the pressure dependence of structural and transport properties of an LixCoO2 single crystal, grown using 5% excess Li in the precursors. Ambient pressure synchrotron diffraction on these crystals reveals that, the excess Li during the growth, has facilitated the stabilization of a layered rhombohedral phase (space group R3m) as well as a disordered rock-salt phase (space group Fm3m). The volume fraction of the rhombohedral and cubic phase is 60:40, respectively, which remains unchanged up to 10.6 GPa. No structural phase transition has been observed up to 10.6 GPa. An increase in resistance with a decrease in temperature has revealed the semi-metallic nature of the sample. Further, the application of hydrostatic pressure up to 2.8 GPa shows the enhancement of semi-metallic nature. The obtained experimental results can be qualitatively explained via density functional theory (DFT) and thermodynamics modelling. The calculated density of states was reduced, and the activation energy was increased by applied pressure. Our investigations indicate a significant phase stability of the mixed phase crystals under externally applied high pressure and thus suggest the possible use of such mixed phase materials as a cathode in lithium-ion batteries.",2401.11446v1 2017-01-18,Intermittent Preventive Treatment (IPT): Its role in averting disease-induced mortalities in children and in promoting the spread of antimalarial drug resistance,"We develop a variable population age-structured ODE model to investigate the role of Intermittent Preventive Treatment (IPT) in averting malaria-induced mortalities in children, as well as its related cost in promoting the spread of anti-malarial drug resistance. IPT, a malaria control strategy in which a full curative dose of an antimalarial medication is administered to vulnerable asymptomatic individuals at specified intervals, has been shown to have a positive impact on reducing malaria transmission and deaths in children and pregnant women. However, it can also promote drug resistance spread. Our mathematical model is used to explore IPT effects on drug resistance in holoendemic malaria regions while quantifying the benefits in deaths averted. Our model includes both drug-sensitive and drug-resistant strains of the parasite as well as interactions between human hosts and mosquitoes. The basic reproduction numbers for both strains as well as the invasion reproduction numbers are derived and used to examine the role of IPT on drug resistance. Numerical simulations show the individual and combined effects of IPT and treatment of symptomatic infections on the prevalence levels of both parasite strains and on the number of lives saved. The results suggest that while IPT can indeed save lives, particularly in the high transmission region, certain combinations of drugs used for IPT and drugs used to treat symptomatic infection may result in more deaths when resistant parasite strains are circulating. Moreover, the half-lives of the treatment and IPT drugs used play an important role in the extent to which IPT may influence the rate of spread of the resistant strain. A sensitivity analysis indicates the model outcomes are most sensitive to the reduction factor of transmission for the resistant strain, rate of immunity loss, and the clearance rate of sensitive infections.",1701.05210v1 2019-12-22,Bulk Polycrystalline Ceria Doped Al$_2$O$_3$ and YAG Ceramics for High-Power Density Laser-Driven Solid-State White Lighting: Effects of Crystallinity and Extreme Temperatures,"Here we develop and characterize high thermal conductivity/high thermal shock resistant bulk Ce doped Al2O3 and propose it as a new phosphor converting capping layer for high-powered/high-brightness solid-state white lighting (SSWL). The bulk, dense Ce:Al2O3 ceramics have a 0.5 at.% Ce:Al concentration (significantly higher than the equilibrium solubility limit), and were produced using a simultaneous solid-state reactive Current Activated Pressure-Assisted Densification (CAPAD) approach. Ce:Al2O3 exhibits a broadband emission from 400-600nm, which encompasses the entire blue and green portions of the visible spectrum when pumped with ultra-violet (UV) light that is now commercially available in UV light emitting devices (LED) and laser diodes (LD). These broadband phosphors can be used in the commonly employed scheme of mixing with other UV converting capping layers that emit red light to produce white light. Alternatively, they can be used in a novel composite down converter approach that ensures improved thermal-mechanical properties of the converting phosphor capping layer. In this configuration Ce:Al2O3 is used with proven phosphor conversion materials such as Ce:YAG as an active encapsulant or as a capping layer to produce SSWL with an improved bandwidth in the blue portion of the visible spectrum. In order to study the effect of crystallinity on the Ce PL emission, we synthesize Ce:YAG ceramics using high-pressure CAPAD at moderate temperatures to obtain varying crystallinity (amorphous through fully -crystalline). We investigate the PL characteristics of Ce:Al2O3 and Ce:YAG from 295K to 4K, revealing unique crystal field effects from the matrix on the Ce-dopants. The unique PL properties in conjunction with the superior thermal-mechanical properties of Ce:Al2O3 can be used in high-powered/high-brightness integrated devices based on high-efficiency UV-LD that do not suffer",1912.10393v1 1992-08-05,Transport Properties of the Infinite Dimensional Hubbard Model,"Results for the optical conductivity and resistivity of the Hubbard model in infinite spatial dimensions are presented. At half filling we observe a gradual crossover from a normal Fermi-liquid with a Drude peak at $\omega=0$ in the optical conductivity to an insulator as a function of $U$ for temperatures above the antiferromagnetic phase transition. When doped, the ``insulator'' becomes a Fermi-liquid with a corresponding temperature dependence of the optical conductivity and resistivity. We find a $T^2$-coefficient in the low temperature resistivity which suggests that the carriers in the system acquire a considerable mass-enhancement due to the strong local correlations. At high temperatures, a crossover into a semi-metallic regime takes place.",9208002v1 1997-12-05,Spin flip scattering in magnetic junctions,"Processes which flip the spin of an electron tunneling in a junction made up of magnetic electrodes are studied. It is found that: i) Magnetic impurities give a contribution which increases the resistance and lowers the magnetoresistance, which saturates at low temperatures. The conductance increases at high fields. ii) Magnon assisted tunneling reduces the magnetoresistance as $T^{3/2}$, and leads to a non ohmic contribution to the resistance which goes as $V^{3/2}$, iii) Surface antiferromagnetic magnons, which may appear if the interface has different magnetic properties from the bulk, gives rise to $T^2$ and $V^2$ contributions to the magnetoresistance and resistance, respectively, and, iv) Coulomb blockade effects may enhance the magnetoresistance, when transport is dominated by cotunneling processes.",9712075v1 1998-12-14,Charged impurity scattering limited low temperature resistivity of low density silicon inversion layers,"We calculate within the Boltzmann equation approach the charged impurity scattering limited low temperature electronic resistivity of low density $n$-type inversion layers in Si MOSFET structures. We find a rather sharp quantum to classical crossover in the transport behavior in the $0 - 5$K temperature range, with the low density, low temperature mobility showing a strikingly strong non-monotonic temperature dependence, which may qualitatively explain the recently observed anomalously strong temperature dependent resistivity in low-density, high-mobility MOSFETs.",9812216v3 2000-02-17,"Strong, Ultra-narrow Peaks of Longitudinal and Hall Resistances in the Regime of Breakdown of the Quantum Hall Effect","With unusually slow and high-resolution sweeps of magnetic field, strong, ultra-narrow (width down to $100 {\rm \mu T}$) resistance peaks are observed in the regime of breakdown of the quantum Hall effect. The peaks are dependent on the directions and even the history of magnetic field sweeps, indicating the involvement of a very slow physical process. Such a process and the sharp peaks are, however, not predicted by existing theories. We also find a clear connection between the resistance peaks and nuclear spin polarization.",0002267v1 2001-03-28,Microwave Surface Resistance in MgB2,"Measurements of the temperature dependence of the surface resistance at 3 GHz of 100 micron size grains of MgB_2 separated powder are presented and discussed. The microwave surface resistance data is compared to experimental results of Nb, Bi_2Sr_2CaCu_2O_{8+\delta} (BSCCO) and theoretical predictions of s-wave weak coupling electron-phonon theory (BCS).",0103587v2 2002-10-17,Origin of superconductivity transition broadening in MgB2,"We report resistivity and magnetization of single crystal MgB2, focusing on the broadening of superconducting (SC) transition in magnetic fields. In-plane and out-of-plane resistivity indicate that the broadening of superconducting transition is independent of Lorentz force and that it is merely dependent on the magnetic field direction. In magnetization, diamagnetic signal begins to appear at almost the same temperature as the onset temperature of resistivity transition. These results suggest that the broadening is attributed not to the surface superconductivity but to the superconducting fluctuation or the vortex-liquid picture, owing to the short coherence length and the high transition temperature of MgB2.",0210358v1 2003-03-07,Drift plasma instability near the edge as the origin of the microwave-induced zero-resistance states,"We discuss a possible origin of the recently discovered microwave-induced zero-resistance states in very-high-electron-mobility two-dimensional electron systems. We suggest a scenario, in which two mechanisms, bulk and edge, contribute to the measured photosignal. Zero-resistance states are assumed to be due to a drift plasma instability, developing {\em near the edge} of the system under the microwave radiation. The proposed scheme qualitatively agrees with the microwave power, temperature, frequency, magnetic field, and mobility dependencies of the measured photosignal.",0303130v1 2003-04-22,Upper critical fields of MgB2 thin films,"Critical fields of four MgB2 thin films with a normal state resistivity ranging from 5 to 50 mWcm and Tc from 29.5 to 38.8 K were measured up to 28 T. Hc2(T) curves present a linear behavior towards low temperatures. Very high critical field values have been found, up to 24 T along the c-axis and 57 T in the basal plane not depending on the normal state resistivity values. In this paper, critical fields will be analyzed taking into account the multiband nature of MgB2; we will show that resistivity and upper critical fields can be ascribed to different scattering mechanisms.",0304478v1 2004-07-14,Zero-Resistance States Induced by Electromagnetic-Wave Excitation in GaAs/AlGaAs Heterostructures,"We report the detection of novel zero-resistance states induced by electromagnetic wave excitation in ultra high mobility GaAs/AlGaAs heterostructure devices, at low magnetic fields, $B$, in the large filling factor limit. Vanishing resistance is observed in the vicinity of $B = [4/(4j+1)] B_{f}$, where $B_{f} = 2\pi\textit{f}m^{*}/e$, where m$^{*}$ is the effective mass, e is the charge, and \textit{f} is the microwave frequency. The dependence of the effect is reported as a function of \textit{f}, the temperature, and the power.",0407367v1 2006-04-03,Pulsed versus DC I-V characteristics of resistive manganites,"We report on pulsed and DC I-V characteristics of polycrystalline samples of three charge-ordered manganites, Pr_{2/3}Ca_{1/3}MnO_3, Pr_{1/2}Ca_{1/2}MnO_3, Bi_{1/2}Sr_{1/2}MnO_3 and of a double-perovskite Sr_2MnReO_6, in a temperature range where their ohmic resistivity obeys the Efros-Shklovskii variable range hopping relation. For all samples, the DC I(V) exhibits at high currents negative differential resistance and hysteresis, which mask a perfectly ohmic or a moderately nonohmic conductivity obtained by pulsed measurements. This demonstrates that the widely used DC I-V measurements are usually misleading.",0604049v1 2006-06-13,Peculiar behavior of the electrical resistivity of MnSi at the ferromagnetic phase transition,"The electrical resistivity of a single crystal of MnSi was measured across its ferromagnetic phase transition line at ambient and high pressures. Sharp peaks of the temperature coefficient of resistivity characterize the transition line. Analysis of these data shows that at pressures to ~0.35 GPa these peaks have fine structure, revealing a shoulder at ~ 0.5 K above the peak. It is symptomatic that this structure disappears at pressures higher than ~0.35 GPa, which was identified earlier as a tricritical point",0606324v1 2006-10-23,Microwave induced negative resistance states in 2D electron gas with periodic modulation,"We study the microwave-induced photoconductivity of a two-dimensional electron system (2DES) in the presence of a magnetic field and a two-dimensional modulation. The microwave and Landau contributions are exactly taken into account, while the periodic potential is treated perturbatively. The longitudinal resistivity exhibits oscillations, periodic in $\omega / \omega_c$. Negative resistance states (NRS) develop for sufficiently high electron mobility and microwave power. This phenomenon appears in a narrow window region of values of the lattice parameter ($a$), around $a \sim l_B$, where $l_B$ is the magnetic length. It is proposed that these phenomena may be observed in artificially fabricated arrays of periodic scatterers at the interface of ultraclean heterostructures. {73.20.At,05.60.-k, 72.15.Rn}",0610643v1 2002-09-10,"Evolution of Electrical Resistivity, Thermal Conductivity, and Temperature of a solid under the action of Intense Ultrashort Laser pulse","The dynamical properties of Cu in a regime relevant to femtosecond micro machining are obtained on picosecond time scales using pump-probe reflectivity study for 100fs, 1015 W cm-2 laser pulses. The electrical resistivity is obtained by solving Helmoltz equations. The dissipation mechanisms and scaling laws are obtained in high and low temperature limits. The 'resistivity saturation' effect in an unexplored regime intermediate to hot plasma and cold solid is studied in detail. The temperature evolution and thermal conductivity is obtained in the temporal range 0 to 30ps after the interaction of laser pulse with solid Cu.",0209037v1 1996-07-12,Flux flow resistivity and vortex viscosity of high-Tc films,"The flux flow regime of high-T$_{\rm c}$ samples of different normal state resistivities is studied in the temperature range where the sign of the Hall effect is reversed. The scaling of the vortex viscosity with normal state resistivity is consistent with the Bardeen-Stephen theory. Estimates of the influence of possible mechanisms suggested for the sign reversal of the Hall effect are also given.",9607003v1 2007-05-15,Excitation of MHD waves in magnetized anisotropic cosmologies,"The excitation of cosmological perturbations in an anisotropic cosmological model and in the presence of a homogeneous magnetic field was studied, using the resistive magnetohydrodynamic (MHD) equations. We have shown that fast-magnetosonic modes, propagating normal to the magnetic field grow exponentially and saturated at high values, due to the resistivity. We also demonstrate that the jeans-like instabilities are enhanced inside a resistive and the formation of condensations formed within an anisotropic fluid influence the growing magnetosonic waves.",0705.2194v1 2007-12-10,Non-local electron transport and cross-resistance peak in NSN heterostructures,"We develop a microscopic theory describing the peak in the temperature dependence of the non-local resistance of three-terminal NSN devices. This peak emerges at sufficiently high temperatures as a result of a competition between quasiparticle/charge imbalance and subgap (Andreev) contributions to the conductance matrix. Both the height and the shape of this peak demonstrate the power law dependence on the superconductor thickness $L$ in contrast to the zero-temperature non-local resistance which decays (roughly) exponentially with increasing $L$. A similar behavior was observed in recent experiments.",0712.1408v1 2008-10-08,Pressure-induced superconductivity in Iron pnictide compound SrFe2As2,"Electrical resistivity under high pressure have been measured on nominally pure SrFe2As2 up to 14 GPa. The resistivity drop appeared with increasing pressure, and we clearly observed zero resistivity. The maximum of superconducting transition temperature (Tc) is 38 K. The value is corresponding to the one of optimally doping AFe2As2 (A=Sr, Ba) system with K+ ions at the A2+ site.",0810.1377v1 2010-12-13,Role of domain wall fluctuations in non-Fermi liquid behavior of metamagnets,"We study resistivity temperature dependence of a three dimensional metamagnet near the metamagnet phase transition point in the case when magnetic structure tends to split into regions with high and low magnetization. We show that in the case of weak pinning the spin relaxation time of domain wall is much larger than that of the volume spin fluctuations. This opens a temperature range where resistivity temperature dependence is determined by scattering of conducting electrons by the domain wall fluctuations. We show that it leads to quasi-linear low temperature dependence of resistivity.",1012.2617v2 2011-09-04,Phase diffusion in graphene-based Josephson junctions,"We report on graphene-based Josephson junctions with contacts made from lead. The high transition temperature of this superconductor allows us to observe the supercurrent branch at temperatures up to $\sim 2$ K, at which point we can detect a small, but non-zero, resistance. We attribute this resistance to the phase diffusion mechanism, which has not been yet identified in graphene. By measuring the resistance as a function of temperature and gate voltage, we can further characterize the nature of electromagnetic environment and dissipation in our samples.",1109.0769v1 2012-12-01,Modeling magnetized neutron stars using resistive MHD,"This work presents an implementation of the resistive MHD equations for a generic algebraic Ohm's law which includes the effects of finite resistivity within full General Relativity. The implementation naturally accounts for magnetic-field-induced anisotropies and, by adopting a phenomenological current, is able to accurately describe electromagnetic fields in the star and in its magnetosphere. We illustrate the application of this approach in interesting systems with astrophysical implications; the aligned rotator solution and the collapse of a magnetized rotating neutron star to a black hole.",1212.0130v1 2013-06-29,On the beneficial role of noise in resistive switching,"We study the effect of external noise on resistive switching. Experimental results on a manganite sample are presented showing that there is an optimal noise amplitude that maximizes the contrast between high and low resistive states. By means of numerical simulations, we study the causes underlying the observed behavior. We find that experimental results can be related to general characteristics of the equations governing the system dynamics.",1307.0143v1 2015-01-22,Tests of a Novel Design of Resistive Plate Chambers,"A novel design of Resistive Plate Chambers (RPCs), using only a single resistive plate, is being proposed. Based on this design, two large size prototype chambers were constructed and were tested with cosmic rays and in particle beams. The tests confirmed the viability of this new approach. In addition to showing an improved single-particle response compared to the traditional 2-plate design, the novel chambers also prove to be suitable for calorimetric applications.",1501.05907v2 2015-10-12,Radiation-assisted magnetotransport in two-dimensional electron gas systems: appearance of zero resistance states,"Zero-Resistance States (ZRS) are normally associated with superconducting and quantum Hall phases. Experimental detection of ZRS in two-dimensional electron gas (2DEG) systems irridiated by microwave(MW) radiation in a magnetic field has been quite a surprise. We develop a semiclassical transport formalism to explain the phenomena. We find a sequence of Zero-Resistance States (ZRS) inherited from the suppression of Shubnikov-de Haas (SdH) oscillations under the influence of high-frequency and large amplitude microwave radiation. Furthermore, the ZRS are well pronounced and persist up to broad intervals of magnetic field as observed in experiments on microwave illuminated 2DEG systems.",1510.03187v1 2016-06-27,"Characterization of Methicillin-resistant Staphylococcus aureus Isolates from Fitness Centers in Memphis Metropolitan Area, USA","Indoor skin-contact surfaces of public fitness centers may serve as reservoirs of potential human transmission of methicillin-resistant Staphylococcus aureus (MRSA). We found a high prevalence of multi-drug resistant (MDR)-MRSA of CC59 lineage harboring a variety of extracellular toxin genes from surface swab samples collected from inanimate surfaces of fitness centers in Memphis metropolitan area, USA. Our findings underscore the role of inanimate surfaces as potential sources of transmission of MDR-MRSA strains with considerable genetic diversity.",1606.08377v1 2017-08-18,Map-based cloning of the gene Pm21 that confers broad spectrum resistance to wheat powdery mildew,"Common wheat (Triticum aestivum L.) is one of the most important cereal crops. Wheat powdery mildew caused by Blumeria graminis f. sp. tritici (Bgt) is a continuing threat to wheat production. The Pm21 gene, originating from Dasypyrum villosum, confers high resistance to all known Bgt races and has been widely applied in wheat breeding in China. In this research, we identify Pm21 as a typical coiled-coil, nucleotide-binding site, leucine-rich repeat gene by an integrated strategy of resistance gene analog (RGA)-based cloning via comparative genomics, physical and genetic mapping, BSMV-induced gene silencing (BSMV-VIGS), large-scale mutagenesis and genetic transformation.",1708.05475v1 2021-04-27,Unified description of resistivity and thermopower of Pr$_2$Ir$_2$O$_7$: possible influence of crystal field excitation in a Kondo lattice,"We present experimental evidence of incoherent Kondo scattering as the source of resistivity minima in bulk polycrystalline and nanocrystalline Pr$_2$Ir$_2$O$_7$. The temperature dependence of thermopower shows a positive maximum at high temperature followed by a negative minimum at low temperature, with the sign inversion occurring at a much higher temperature than $T_K$. Moreover, we observe little correlation between TK and intersite coupling strength given by $\theta_{CW}$. We describe the temperature dependence of thermopower and resistivity within the framework of crystal field excitation in a Kondo lattice.",2105.05149v1 2022-05-03,On the problem of projectile motion in a medium with quadratic resistance,"A classic problem of the motion of a projectile thrown at an angle to the horizon in a medium with a quadratic resistance law is studied. An approximate analytical solution of the equations of projectile motion is presented, which has a high accuracy. The proposed formulas are universal, that is, they can be used for any initial conditions of throwing over a wide range of the change of medium resistance coefficient. The motion of a shuttlecock of badminton, bullet, table tennis ball and volleyball are presented as examples.",2205.01564v1 2013-08-15,Structural and optical investigations of the iron-chalcogenide superconductor Fe$_{1.03}$Se$_{0.5}$Te$_{0.5}$ under high pressure,"Iron-chalcogenide superconductor Fe$_{1.03}$Se$_{0.5}$Te$_{0.5}$ has been investigated under high pressure using synchrotron based x-ray diffraction and mid-infrared reflectance measurements at room temperature. Pressure dependence of the superconducting transition temperature (T$_c$) of the same sample has been determined by temperature-dependent resistance measurements up to 10 GPa. Although the high pressure orthorhombic phase ($\textit{Pbnm}$) starts emerging at 4 GPa, structural transition becomes clearly observable above 10 GPa. A strong correlation is observed between the Fe(Se,Te)$_{4}$ tetrahedral deformation in the tetragonal phase ($\textit{P4/nmm}$) and the sharp rise of T$_c$ up to $\sim$4 GPa, above which T$_c$ is found to be almost pressure independent at least up to 10 GPa. A subtle structural modification of the tetragonal phase is noticed above 10 GPa, suggesting a structural transition with possible Fe$^{2+}$ spin-state transition. The evolution with pressure of the optical conductivity shows that the Drude term increases systematically with pressure up to 5.4 GPa, indicating the evolution of the tetragonal phase towards a conventional metallic state. At further higher pressures the Drude term reduces drastically implying a poor metallic character of the high pressure orthorhombic phase. Our results suggest that occurrence of large onset T$_c$ above 4 GPa is due to a systematic increase of high pressure orthorhombic phase fraction.",1308.3367v1 2016-07-11,High pressure studies on properties of FeGa3: role of on-site coulomb correlation,"High pressure X-ray diffraction measurements have been carried out on the intermetallic semiconductor FeGa$_3$ and the equation of state for FeGa$_3$ has been determined. First principles based DFT calculations within the GGA approximation indicate that although the unit cell volume matches well with the experimentally obtained value at ambient pressure, it is significantly underestimated at high pressures and the difference between them increases as pressure increases. GGA + U calculations with increasing values of U$_{Fe(3d)}$ (on-site Coulomb repulsion between the Fe 3d electrons) at high pressures, correct this discrepancy. Further, the GGA+U calculations also show that along with U$_{Fe(3d)}$, the Fe 3d band width also increases with pressure and around a pressure of 4 GPa, a small density of states appear at the Fermi level. High pressure resistance measurements carried out on FeGa$_3$ also clearly show a signature of an electronic transition. Beyond the pressure of 19.7 GPa, the diffraction peaks reduce in intensity and are not observable beyond $\sim$ 26 GPa, leading to an amorphous state.",1607.02905v2 2016-10-24,Deep Reactive Ion Etched Anti-Reflection Coatings for Sub-millimeter Silicon Optics,"Refractive optical elements are widely used in millimeter and sub-millimeter astronomical telescopes. High resistivity silicon is an excellent material for dielectric lenses given its low loss-tangent, high thermal conductivity and high index of refraction. The high index of refraction of silicon causes a large Fresnel reflectance at the vacuum-silicon interface (up to 30%), which can be reduced with an anti-reflection (AR) coating. In this work we report techniques for efficiently AR coating silicon at sub-millimeter wavelengths using Deep Reactive Ion Etching (DRIE) and bonding the coated silicon to another silicon optic. Silicon wafers of 100 mm diameter (1 mm thick) were coated and bonded using the Silicon Direct Bonding technique at high temperature (1100 C). No glue is used in this process. Optical tests using a Fourier Transform Spectrometer (FTS) show sub-percent reflections for a single-layer DRIE AR coating designed for use at 320 microns on a single wafer. Cryogenic (10 K) measurements of a bonded pair of AR-coated wafers also reached sub-percent reflections. A prototype two-layer DRIE AR coating to reduce reflections and increase bandwidth is presented and plans for extending this approach are discussed.",1610.07655v1 2020-03-09,CACTUS: A depleted monolithic active timing sensor using a CMOS radiation hard technology,"The planned luminosity increase at the Large Hadron Collider in the coming years has triggered interest in the use of the particles' time of arrival as additional information in specialized detectors to mitigate the impact of pile-up. The required time resolution is of the order of tens of picoseconds, with a spatial granularity of the order of 1 mm. A time measurement at this precision level will also be of interest beyond the LHC and beyond high energy particle physics. We present in this paper the first developments towards a radiation hard Depleted Monolithic Active Pixel Sensor (DMAPS), with high-resolution time measurement capability. The technology chosen is a standard high voltage CMOS process, in conjunction with a high resistivity detector material, which has already proven to efficiently detect particles in tracking applications after several hundred of Mrad of irradiation.",2003.04102v4 2019-02-23,Pixel detector R&D for the Compact Linear Collider,"The physics aims at the proposed future CLIC high-energy linear $e^+ e^-$ collider pose challenging demands on the performance of the detector system. In particular the vertex and tracking detectors have to combine precision measurements with robustness against the expected high rates of beam-induced backgrounds. A spatial resolution of a few microns and a material budget down to 0.2\% of a radiation length per vertex-detector layer have to be achieved together with a few nanoseconds time stamping accuracy. These requirements are addressed with innovative technologies in an ambitious detector R\&D programme, comprising hardware developments as well as detailed device and Monte Carlo simulations based on TCAD, Geant4 and Allpix-Squared. Various fine pitch hybrid silicon pixel detector technologies are under investigation for the CLIC vertex detector. The CLICpix and CLICpix2 readout ASICs with \SI{25}{\micro\meter} pixel pitch have been produced in a \SI{65}{\nano\meter} commercial CMOS process and bump-bonded to planar active edge sensors as well as capacitively coupled to High-Voltage (HV) CMOS sensors. Monolithic silicon tracking detectors are foreseen for the large surface ($\approx$ \SI{140}{\meter\squared}) CLIC tracker. Fully monolithic prototypes are currently under development in High-Resistivity (HR) CMOS, HV-CMOS and Silicon on Insulator (SOI) technologies. The laboratory and beam tests of all recent prototypes profit from the development of the CaRIBou universal readout system. This talk presents an overview of the CLIC pixel-detector R\&D programme, focusing on recent test-beam and simulation results.",1902.08752v4 2017-05-30,Structural evolution of CO2 filled pure silica LTA zeolite under high-pressure high-temperature conditions,"The crystal structure of CO2 filled pure SiO2 LTA zeolite has been studied at high pressures and temperatures using synchrotron based x ray powder diffraction. Its structure consists of 13 CO2 guest molecules, 12 of them accommodated in the large alpha cages and 1 in the beta cages, giving a SiO2:CO2 stoichiometric ratio smaller than 2. The structure remains stable under pressure up to 20 GPa with a slight pressure dependent rhombohedral distortion, indicating that pressure induced amorphization is prevented by the insertion of guest species in this open framework. The ambient-temperature lattice compressibility has been determined. In situ high pressure resistive heating experiments up to 750 K allow us to estimate the thermal expansivity at 5 GPa. Our data confirm that the insertion of CO2 reverses the negative thermal expansion of the empty zeolite structure. No evidence of any chemical reaction was observed. The possibility of synthesizing a silicon carbonate at high temperatures and higher pressures is discussed in terms of the evolution of C-O and Si-O distances between molecular and framework atoms.",1705.10507v1 2018-08-22,Record-High Superconductivity in Niobium-Titanium Alloy,"Here we report the observation of extraordinary superconductivity in a pressurized commercial niobium-titanium alloy. We find that its zero-resistance superconductivity persists from ambient pressure to the pressure as high as 261.7 GPa, a record high pressure up to which a known superconducting state can continuously survives. Remarkably, at such an ultra-high pressure, although the ambient pressure volume is shrunk by 45% without structural phase transition, the superconducting transition temperature (TC) increases to ~19.1 K from ~9.6 K, and the critical magnetic field (HC2) at 1.8 K has been enhanced to 19 T from 15.4 T. These results set new records for both of the TC and the HC2 among all the known alloy superconductors composed of only transition metal elements. The remarkable high pressure superconducting properties observed in the NbTi alloy not only expand our knowledge on this important commercial superconductor but also are helpful for a better understanding on the superconducting mechanism.",1808.07215v3 2022-09-02,Ultra-Low Temperature Li/CFx Batteries Enabled by Fast-transport and Anion-pairing Liquefied Gas Electrolytes,"Lithium fluorinated carbon is one of the most promising chemistries for high-energy-density primary energy storage systems in applications where rechargeability is not required. Though Li/CFx demonstrates high energy density under ambient conditions, achieving such a high energy density when exposed to subzero temperatures remains a challenge, particularly under high current density. Here, we report a liquefied gas electrolyte with an anion-pair solvation structure based on dimethyl ether with a low melting point and low viscosity, leading to high ionic conductivity between a wide temperature range. Besides that, through systematic X-ray photoelectron spectroscopy integrated with transmission electron microscopy characterizations, we evaluate the interface of CFx for low-temperature performance. We conclude that the fast transport and anion-pairing solvation structure of the electrolyte bring about reduced charge transfer resistance at low temperatures, which resulted in significantly enhanced performance of Li/CFx cells. Utilizing 50 mg/cm2 loading electrodes, the Li/CFx still displayed 1530 Wh/kg at reduced temperature. This work provides insights into the electrolyte design that may overcome the operational limits of batteries in extreme environments.",2209.02409v1 2023-03-09,Superconductivity above 70 K observed in lutetium polyhydrides,"The binary polyhydrides of heavy rare earth lutetium that shares a similar valence electron configuration to lanthanum have been experimentally discovered to be superconductive. The lutetium polyhydrides were successfully synthesized at high pressure and high temperature conditions using a diamond anvil cell in combinations with the in-situ high pressure laser heating technique. The resistance measurements as a function of temperature were performed at the same pressure of synthesis in order to study the transitions of superconductivity (SC). The superconducting transition with a maximum onset temperature (Tc) 71 K was observed at pressure of 218 GPa in the experiments. The Tc decreased to 65 K when pressure was at 181 GPa. From the evolution of SC at applied magnetic fields, the upper critical field at zero temperature {\mu}0Hc2(0) was obtained to be ~36 Tesla. The in-situ high pressure X-ray diffraction experiments imply that the high Tc SC should arise from the Lu4H23 phase with Pm-3n symmetry that forms a new type of hydrogen cage framework different from those reported for previous light rare earth polyhydride superconductors.",2303.05117v3 2023-04-04,Ultrathin Stable Ohmic Contacts for High-Temperature Operation of $β$-Ga$_2$O$_3$ Devices,"Beta gallium oxide ($\beta$-Ga$_2$O$_3$) shows significant promise in the high-temperature, high-power, and sensing electronics applications. However, long-term stable metallization layers for Ohmic contacts at high temperature present unique thermodynamic challenges. The current most common Ohmic contact design based on 20 nm of Ti has been repeatedly demonstrated to fail at even moderately elevated temperatures (300-400$^{\circ}$C) due to a combination of non-stoichiometric Ti/Ga$_2$O$_3$ interfacial reactions and kinetically favored Ti diffusion processes. Here we demonstrate stable Ohmic contacts for Ga$_2$O$_3$ devices operating up to 500-600$^{\circ}$C using ultrathin Ti layers with a self-limiting interfacial reaction. The ultrathin Ti layer in the 5nm Ti / 100nm Au contact stack is designed to fully oxidize while forming an Ohmic contact, thereby limiting both thermodynamic and kinetic instability. This novel contact design strategy results in an epitaxial conductive anatase titanium oxide interface layer that enables low-resistance Ohmic contacts that are stable both under long-term continuous operation (>500 hours) at 600$^{\circ}$C in vacuum ($\leq$ 10$^{-4}$ Torr), as well as after repeated thermal cycling (15 times) between room temperature and 550$^{\circ}$C in flowing N$_2$. This stable Ohmic contact design will accelerate the development of high-temperature devices by enabling research focus to shift towards rectifying contacts and other interfacial layers.",2304.02161v1 2023-07-31,Coexistence of Superconductivity and ferromagnetism in high entropy carbide ceramics,"Generally, the superconductivity was expected to be absent in magnetic systems, but this reception was disturbed by unconventional superconductors, such as cuprates, iron-based superconductors and recently discovered nickelate, since their superconductivity is proposed to be related to the electron-electron interaction mediated by the spin fluctuation. However, the coexistence of superconductivity and magnetism is still rare in conventional superconductors. In this work, we reported the coexistence of these two quantum orderings in high entropy carbide ceramics (Mo0.2Nb0.2Ta0.2V0.2W0.2)C0.9, (Ta0.25Ti0.25Nb0.25Zr0.25)C, and they are expected to be conventional superconductors. Clear magnetic hysteresis loop was observed in these high entropy carbides, indicating a ferromagnetic ground state. A sharp superconducting transition is observed in (Mo0.2Nb0.2Ta0.2V0.2W0.2)C0.9 with a Tc of 3.4 K and upper critical field of ~3.35 T. Meanwhile, superconductivity is suppressed to some extent and zero-resistance state disappears in (Ta0.25Ti0.25Nb0.25Zr0.25)C, in which stronger magnetism is presented. The upper critical field of (Ta0.25Ti0.25Nb0.25Zr0.25)C is only ~1.5 T, though they show higher transition temperature near 5.7 K. The ferromagnetism stems from the carbon vacancies which occurs often during the high temperature synthesis process. This work not just demonstrate the observation of superconductivity in high entropy carbide ceramics, but also provide alternative exotic platform to study the correlation between superconductivity and magnetism, and is of great benefit for the design of multifunctional electronic devices.",2307.16438v1 2023-09-09,High-speed metasurface modulator using critically coupled bimodal plasmonic resonance,"Free-space electro-optic (EO) modulators operating at gigahertz and beyond are attractive for a wide range of emerging applications, including high-speed imaging, free-space optical communication, microwave photonics, and diffractive computing. Here we experimentally demonstrate a high-speed plasmonic metasurface EO modulator operating at a near-infrared wavelength range with a gigahertz modulation bandwidth. To achieve efficient intensity modulation of reflected light from an ultrathin metasurface layer, we utilize the bimodal plasmonic resonance inside a subwavelength metal-insulator-metal grating, which is precisely tuned to satisfy the critical coupling condition. As a result, perfect absorption of -27 dB (99.8%) and a high quality (Q) factor of 113 are obtained at a resonant wavelength of 1650 nm. By incorporating an EO polymer inside the grating, we achieve a modulation depth of up to 9.5 dB under an applied voltage of $\pm$30 V. The 3-dB modulation bandwidth is confirmed to be 1.25 GHz, which is primarily limited by the undesired contact resistance. Owing to the high electrical conductivity of metallic gratings and a compact device structure with a minimal parasitic capacitance, the demonstrated device can potentially operate at several tens of gigahertz, which opens up exciting opportunities for ultrahigh-speed active metasurface devices in various applications.",2309.04835v1 2000-07-10,"Comment on ""Microwave vortex dissipation of superconducting Nd-Ce-Cu-O epitaxial films in high magnetic fields""","While the electrodynamic treatment of a superconducting thin film by Yeh et al. [Phys. Rev. B 48, 9861 (1993)] ostensibly has application for the ""thin-film limit,"" their work is shown to employ bulk-like instead of thin-film electrodynamics, and as such obtains an ostensible violation of the first law of thermodynamics and a surface resistance independent of the resistivity. Other theoretical and experimental difficulties are briefly noted.",0007167v1 2000-10-27,Negative differential resistance in nanotube devices,"Carbon nanotube junctions are predicted to exhibit negative differential resistance, with very high peak-to-valley current ratios even at room temperature. We treat both nanotube p-n junctions and undoped metal-nanotube-metal junctions, calculating quantum transport through the self-consistent potential within a tight-binding approximation. The undoped junctions in particular may be suitable for device integration.",0010456v1 2002-05-20,Resistive Transition Equation of Mixed State,"We present a microscopic derivation of the resistive transition equation for mixed state of superconductors. This form fits the experimental data of MgB2 with parameters in agreement with the prediction of BCS superconductivity. It also fits the experimental data of high quality untwined YBCO single crystal but with parameters somewhat different from the BCS prediction. A discussion in connection with the problem of cuprate superconductivity is given.",0205407v1 2005-04-08,Photo-excited zero-resistance states in the GaAs/AlGaAs system,"The microwave-excited high mobility two-dimensional electron system exhibits, at liquid helium temperatures, vanishing resistance in the vicinity of $B = [4/(4j+1)] B_{f}$, where $B_{f} = 2\pi\textit{f}m^{*}/e$, m$^{*}$ is an effective mass, e is the charge, and \textit{f} is the microwave frequency. Here, we summarize some experimental results.",0504206v1 2009-12-09,2-D MHD Configurations for Accretion Disks Around Magnetized Stars,"We discuss basic features of steady accretion disk morphology around magnetized compact astrophysical objects. A comparison between the standard model of accretion based on visco-resistive MHD and the plasma instabilities, like ballooning modes, triggered by very low value of resistivity, is proposed.",0912.1721v1 2021-06-18,The effect of viscosity and resistivity on Rayleigh-Taylor instability induced mixing in magnetized high energy density plasmas,"This work numerically investigates the role of viscosity and resistivity on Rayleigh-Taylor instabilities in magnetized high-energy-density (HED) plasmas for a high Atwood number and high plasma beta regimes surveying across plasma beta and magnetic Prandtl numbers. The numerical simulations are performed using the visco-resistive magnetohydrodynamic (MHD) equations. Results presented here show that the inclusion of self-consistent viscosity and resistivity in the system drastically changes the growth of the Rayleigh-Taylor instability (RTI) as well as modifies its internal structure at smaller scales. It is seen here that the viscosity has a stabilizing effect on the RTI. Moreover, the viscosity inhibits the development of small scale structures and also modifies the morphology of the tip of the RTI spikes. On the other hand, the resistivity reduces the magnetic field stabilization supporting the development of small scale structures. The morphology of the RTI spikes is seen to be unaffected by the presence of resistivity in the system. An additional novelty of this work is in the disparate viscosity and resistivity profiles that may exist in HED plasmas and their impact on RTI growth, morphology, and the resulting turbulence spectra. Furthermore, this work shows that the dynamics of the magnetic field is independent of viscosity and likewise the resistivity does not affect the dissipation of enstrophy and kinetic energy. In addition, power-law scalings of enstrophy, kinetic energy, and magnetic field energy are provided in both injection range and inertial sub-range which could be useful for understanding RTI induced turbulent mixing in HED laboratory and astrophysical plasmas and could aid in the interpretation of observations of RTI-induced turbulence spectra.",2106.10391v2 2003-03-20,Current-induced phase control in charged-ordered Nd0.5Ca0.5MnO3 and Pr0.6Ca0.4MnO3 crystals,"Single crystals of Nd0.5Ca0.5MnO3 and Pr0.6Ca0.4MnO3 show current-induced insulator-metal transitions at low temperatures. In addition, the charge-ordering transition temperature decreases with increasing current. The electroresistive ratio, defined as r0.5/rI where r0.5 is the resistivity at a current of 0.5 mA and rI the resistivity at a given applied current, I, varies markedly with temperature and the value of I. Thermal hysteresis observed in Nd0.5Ca0.5MnO3 and Pr0.6Ca0.4MnO3 at the insulator-metal transition indicates that the transition is first-order. The current-induced changes are comparable to those induced by magnetic fields, and the insulator-metal transition in Pr0.6Ca0.4MnO3 is accordingly associated with a larger drop in resistivity.",0303407v1 2003-07-22,Temperature Dependence of Resistivity of $Sr_2CoMoO_{6-δ}$ Films,"We investigate the temperature dependence of the resistivity and magnetoresistance of a polycrystalline $Sr_2CoMoO_{6-\delta}$ film deposited on (100)-$SrTiO_3$ substrate prepared by the pulsed laser deposition method. X-ray diffraction, Raman and magnetoresistance results demonstrate clearly the coexistence of a ferromagnetic metallic and an antiferromagnetic (or paramagnetic) insulating domain. Percolative transition between these two phases as the temperature varies, which is believed to induce a metal-insulator transition at around $T_C$, has been directly observed in our measurements of the temperature dependence of the sample resistivity. Thus we have provided new direct evidence that a phase separation scenario also exists in the ordered double-perovskite structure materials.",0307527v2 2005-02-13,Transport properties in correlated systems: An analytical model,"Several studies have so far investigated transport properties of strongly correlated systems. Interesting features of these materials are the lack of resistivity saturation well beyond the Mott-Ioffe-Regel limit and the scaling of the resistivity with the hole density in underdoped cuprates. Due to the strongly correlated nature of these materials, mainly numerical techniques have been employed. A key role in this regards is thought to be played by the continuous transfer of spectral weight from coherent to incoherent states. In this paper we employ a simple analytical expression for the electronic Green's function to evaluate both quasi-particle and transport properties in correlated systems. Our analytical approach permits to enlighten the specific role of the spectral transfer due to the correlation on different features. In particular we investigate the dependence of both quasi-particle and transport scattering rate on the correlation degree and the criterion for resistivity saturation. systems.",0502297v3 2005-08-05,Is ZrB12 two gap superconductor?,"We report the measurements of the temperature dependence of the resistivity, \rho(T), magnetic penetration depth,\lambda(T) the lower, Hc1(T), and upper, Hc2(T), critical magnetic fields, for single crystals of dodecaboride ZrB12, diboride ZrB2 and thin films of diboride MgB2. We observe a number of deviations from conventional behavior in these materials. Although ZrB12 behaves like a simple metal in the normal state, the resistive Debye temperature, 300 K, is three times smaller relative to that (800-1200 K) calculated from the specific heat, C(T), data. We observe predominantly quadratic temperature behavior of resistivity in ZrB12 below 25 K, and in ZrB2 below 100 K, indicating the possible importance of the electron-electron interaction in these borides. Superfluid density of ZrB12 displays unconventional temperature dependence with pronounced shoulder at T/Tc equal to 0.65. Contrary to conventional theories we found a linear temperature dependence of Hc2(T) for ZrB12 from Tc down to 0.35 K. We suggest that both \lambda(T) and Hc2(T) dependencies in ZrB12 can be explained by two band BCS model with different superconducting gap and Tc.",0508151v2 2005-10-05,Equipartition of Current in Parallel Conductors on Cooling Through the Superconducting Transition,"Our experiments show that for two or more pieces of a wire, of different lengths in general, combined in parallel and connected to a dc source, the current ratio evolves towards unity as the combination is cooled to the superconducting transition temperature Tc, and remains pinned at that value below it. This re-distribution of the total current towards equipartition without external fine tuning is a surprise. It can be physically understood in terms of a mechanism that involves the flux-flow resistance associated with the transport current in a wire of type-II superconducting material. It is the fact that the flux-flow resistance increases with current that drives the current division towards equipartition.",0510099v3 2006-04-06,Giant magneto-impedance in Ag-doped La0.7Sr0.3MnO3,"The resistive and reactive parts of the magneto-impedance of sintered ferromagnetic samples of La0.7Sr0.3-xAgxMnO3 (x = 0.05, 0.25) have been measured at room temperature (0$, whereas charge fluctuations promote $\Delta\rho<0$, which are both consistent with the doping dependence of $\Delta\rho$ observed in YBa$_{2}$Cu$_{3}$O$_{7}$. We also discuss the role played by CuO chains in these materials, and propose transport experiments in strained HgBa$_{2}$CuO$_{4}$ and Nd$_{2}$CuO$_{4}$ to probe directly the different resistivity anisotropy regimes.",1412.4745v2 2015-01-26,Granularity Controlled Non-Saturating Linear Magneto-resistance in Topological Insulator Bi2Te3 Films,"We report on the magneto-transport properties of chemical vapor deposition grown films of interconnected Bi2Te3 nanoplates. Similar to many other topological insulator (TI) materials, these granular Bi2Te3 films exhibit a linear magneto-resistance (LMR) effect which has received much recent attention. Studying samples with different degree of granularity, we find a universal correlation between the magnitude of the LMR and the average mobility (<\mu>) of the films over nearly two orders of magnitude change of <\mu>. The granularity controlled LMR effect here is attributed to the mobility fluctuation induced classical LMR according to the Parish-Littlewood theory. These findings have implications to both the fundamental understanding and magneto-resistive device applications of TI and small bandgap semiconductor materials.",1501.06497v2 2015-08-20,Atomic Diffusion in the Surface State of Mott Insulator NiS2,"We present resistivity measurements of Mott insulator NiS2 single crystals after heat treatment. We find a strong increase of the low temperature resistivity that relaxes back towards the pristine behaviour over several days with a time constant of 45 h at room temperature. The low temperature resistivity has previously been shown to be dominated by surface conduction (T. Thio and J. Bennett, PRB 50 10574 1994). Consequently, the changes induced by heat treatment are attributed to changes to surface states. Our results suggest the creation of vacancies in the surface that re refilled from the bulk via atomic diffusion. We estimate a diffusion constant of $D \approx 10^{-10}$ m$^2$/s at room temperature. We identify sulphur vacancies as the most likely to form via oxidisation of sulphur forming volatile SO2 during heat treatment. Our results point towards these sulphur vacancies to be the source of surface state localisation in NiS2.",1508.05020v1 2016-11-12,Thermal boundary resistance from transient nanocalorimetry: a multiscale modeling approach,"The Thermal Boundary Resistance at the interface between a nanosized Al film and an Al_{2}O_{3} substrate is investigated at an atomistic level. A room temperature value of 1.4 m^{2}K/GW is found. The thermal dynamics occurring in time-resolved thermo-reflectance experiments is then modelled via macro-physics equations upon insertion of the materials parameters obtained from atomistic simulations. Electrons and phonons non-equilibrium and spatio-temporal temperatures inhomo- geneities are found to persist up to the nanosecond time scale. These results question the validity of the commonly adopted lumped thermal capacitance model in interpreting transient nanocalorimetry experiments. The strategy adopted in the literature to extract the Thermal Boundary Resistance from transient reflectivity traces is revised at the light of the present findings. The results are of relevance beyond the specific system, the physical picture being general and readily extendable to other heterojunctions.",1611.04042v1 2018-01-11,Forbidden Backscattering and Resistance Dip in the Quantum Limit as a Signature for Topological Insulators,"Identifying topological insulators and semimetals often focuses on their surface states, using spectroscopic methods such as angle-resolved photoemission spectroscopy or scanning tunneling microscopy. In contrast, studying the topological properties of topological insulators from their bulk-state transport is more accessible in most labs but seldom addressed. We show that, in the quantum limit of a topological insulator, the backscattering between the only two states on the Fermi surface of the lowest Landau band can be forbidden, at a critical magnetic field. The conductivity is determined solely by the backscattering between the two states, leading to a resistance dip that may serve as a signature for topological insulator phases. More importantly, this forbidden backscattering mechanism for the resistance dip is irrelevant to details of disorder scattering. Our theory can be applied to revisit the experiments on Pb$_{1-x}$Sn$_x$Se, ZrTe$_5$, and Ag$_2$Te families, and will be particularly useful for controversial small-gap materials at the boundary between topological and normal insulators.",1801.03617v3 2018-02-28,Integration of external electric fields in molecular dynamics simulation models for resistive switching devices,"Resistive switching devices emerged a huge amount of interest as promising candidates for non-volatile memories as well as artificial synapses due to their memristive behavior. The main physical and chemical phenomena which define their functionality are driven by externally applied voltages, and the resulting electric fields. Although molecular dynamics simulations are widely used in order to describe the dynamics on the corresponding atomic length and time scales, there is a lack of models which allow for the actual driving force of the dynamics, i.e. externally applied electric fields. This is due to the restriction of currently applied models to either solely conductive, non-reactive or insulating materials, with thicknesses in the order of the potential cutoff radius, i.e., 10 \r{A}. In this work, we propose a generic model, which can be applied in particular to describe the resistive switching phenomena of metal-insulator-metal systems. It has been shown that the calculated electric field and force distribution in case of the chosen example system Cu/a-SiO$_2$/Cu are in agreement with fundamental field theoretical expectations.",1802.10590v4 2018-03-07,Modelling the longitudinal intensity pattern of diffraction resistant beams in stratified media,"In this paper, we study the propagation of the Frozen Wave type beams through non-absorbing stratified media and develop a theoretical method capable to provide the desired spatially shaped diffraction resistant beam in the last material medium. In this context, we also develop a matrix method to deal with stratified media with large number of layers. Additionally, we undertake some discussion about minimizing reflection of the incident FW beam on the first material interface by using thin films. Our results show that it is indeed possible to obtain the control, on demand, of the longitudinal intensity pattern of a diffraction resistant beam even after it undergoes multiple reflections and transmissions at the layer interfaces. Remote sensing, medical and military applications, noninvasive optical measurements, etc., are some fields that can be benefited by the method here proposed.",1803.03529v1 2019-08-22,Non-Thermal Resistive Switching in Mott Insulators,"Resistive switching can be achieved in a Mott insulator by applying current/voltage, which triggers an insulator-metal transition (IMT). This phenomenon is key for understanding IMT physics and developing novel memory elements and brain-inspired technology. Despite this, the roles of electric field and Joule heating in the switching process remain controversial. We resolve this issue by studying nanowires of two archetypical Mott insulators - VO2 and V2O3. Our findings show a crossover between two qualitatively different regimes. In one, the IMT is driven by Joule heating to the transition temperature, while in the other, field-assisted carrier generation gives rise to a doping driven IMT which is purely non-thermal. By identifying the key material properties governing these phenomena, we propose a universal mechanism for resistive switching in Mott insulators. This understanding enabled us to control the switching mechanism using focused ion-beam irradiation, thereby facilitating an electrically driven non-thermal IMT. The energy consumption associated with the non-thermal IMT is extremely low, rivaling that of state of the art electronics and biological neurons. These findings pave the way towards highly energy-efficient applications of Mott insulators.",1908.08555v1 2019-06-06,Training large-scale ANNs on simulated resistive crossbar arrays,"Accelerating training of artificial neural networks (ANN) with analog resistive crossbar arrays is a promising idea. While the concept has been verified on very small ANNs and toy data sets (such as MNIST), more realistically sized ANNs and datasets have not yet been tackled. However, it is to be expected that device materials and hardware design constraints, such as noisy computations, finite number of resistive states of the device materials, saturating weight and activation ranges, and limited precision of analog-to-digital converters, will cause significant challenges to the successful training of state-of-the-art ANNs. By using analog hardware aware ANN training simulations, we here explore a number of simple algorithmic compensatory measures to cope with analog noise and limited weight and output ranges and resolutions, that dramatically improve the simulated training performances on RPU arrays on intermediately to large-scale ANNs.",1906.02698v1 2020-11-03,Thermodynamically Induced Transport Anomaly in Dilute Metals ZrTe$_5$ and HfTe$_5$,"A 40-year-old puzzle in transition metal pentatellurides ZrTe$_5$ and HfTe$_5$ is the anomalous peak in the temperature dependence of the longitudinal resistivity, which is accompanied by sign reverses of the Hall and Seebeck coefficients. We give a plausible explanation for these phenomena without assuming any phase transition or strong interaction effect. We show that due to intrinsic thermodynamics and diluteness of the conducting electrons in these materials, the chemical potential displays a strong dependence on the temperature and magnetic field. With that, we compute resistivity, Hall and Seebeck coefficients in zero field, and magnetoresistivity and Hall resistivity in finite magnetic fields, in all of which we reproduce the main features that are observed in experiments.",2011.01952v2 2020-11-13,Ab initio screening of metallic MAX ceramics for advanced interconnect applications,"The potential of a wide range of layered ternary carbide and nitride MAX phases as conductors in interconnect metal lines in advanced CMOS technology nodes has been evaluated using automated first principles simulations based on density functional theory. The resistivity scaling potential of these compounds, i.e. the sensitivity of their resistivity to reduced line dimensions, has been benchmarked against Cu and Ru by evaluating their transport properties within a semiclassical transport formalism. In addition, their cohesive energy has been assessed as a proxy for the resistance against electromigration and the need for diffusion barriers. The results indicate that numerous MAX phases show promise as conductors in interconnects of advanced CMOS technology nodes.",2011.06902v2 2020-12-02,Interfacial studies in CNT fibre/TiO$_{2}$ photoelectrodes for efficient H$_{2}$ production,"An attractive class of materials for photo(electro)chemical reactions are hybrids based on semiconducting metal oxides and nanocarbons (e.g. carbon nanotubes (CNT), graphene), where the nanocarbon acts as a highly-stable conductive scaffold onto which the nanostructured inorganic phase can be immobilised; an architecture that maximises surface area and minimises charge transport/transfer resistance. TiO$_{2}$/CNT photoanodes produced by atomic layer deposition on CNT fabrics are shown to be efficient for H$_{2}$ production ($0.07 \mu mol/min$ $H_{2}$ at $0.2V$ $vs Ag/AgCl$), nearly doubling the performance of TiO$_{2}$ deposited on planar substrates, with $100 \%$ Faradaic efficiency. The results are rationalised based on electrochemical impedance spectroscopy measurements showing a large reduction in photoelectron transport resistance compared to control samples and a higher surface area. The low TiO$_{2}$/CNT interfacial charge transfer resistance ($10 \Omega$) is consistent with the presence of an interfacial Ti-O-C bond and corresponding electronic hybridisation determined by spatially-resolved Scanning Photoelectron Microscopy (SPEM) using synchrotron radiation.",2012.01109v1 2021-04-26,Role of electron and ion irradiation in a reliable lift-off process with e-beam evaporation and a bilayer PMMA resist system,"This paper addresses issues related to cracking and blisters in deposited films encountered in a lift-off process with electron beam evaporation and a bilayer PMMA resist system. The impact of charged particles, i.e. electrons and ions, is investigated using an electron beam evaporation chamber equipped with ring-magnets and a plate electrode placed in front of the sample. By replacing the plate electrode with a hollow cylinder, the modified evaporation setup utilizing passive components allows a complete elimination of resist shrinkage and blistering yielding near perfect deposition results for a large variety of different materials.",2104.12452v1 2021-05-24,Spatio-temporal dynamics of voltage-induced resistance transition in the double-exchange model,"We present multi-scale dynamical simulations of voltage-induced insulator-to-metal transition in the double exchange model, a canonical example of itinerant magnet and correlated electron systems. By combining nonequilibrium Green's function method with large-scale Landau-Lifshitz-Gilbert dynamics, we show that the transition from an antiferromagnetic insulator to the low-resistance state is initiated by the nucleation of a thin ferromagnetic conducting layer at the anode. The metal-insulator interface separating the two phases is then driven toward the opposite electrode by the voltage stress, giving rise to a growing metallic region. We further show that the initial transformation kinetics is well described by the Kolmogorov-Avrami-Ishibashi model with an effective spatial-dimension that depends on the applied voltage. Implications of our findings for the resistive switching in colossal magnetoresistant materials are also discussed.",2105.11076v2 2021-10-14,Filamentary superconductivity of resistively-switched strontium titanate,"SrTiO$_3$, although a wide gap insulator, has long been known to become metallic and superconducting at extremely low doping levels. This has given rise to questions concerning the coexistence or interdependence of metallicity, superconductivity, and the material's polar properties. This issue becomes especially intriguing in conjunction with the observation that filamentary metallicity can be induced by means of resistive switching at conditions well below relevant doping levels for homogeneous metallicity. In this study, we demonstrate that resistive switching can also be employed to generate superconductivity at the superconducting transition temperature of $T_c$ $\approx$ 0.2 K in SrTiO$_3$. By combining local characterization of the conductivity with theoretical analysis, we propose that the superconducting properties are associated with the electro-formation of columnar-like bundles with a diameter of 40-50 nm, consisting of metallic filaments surrounded by polar regions. We provide a theoretical model identifying the coexistence of metallic and polar regions as a prerequisite for the filamentary-like superconductivity observed.",2110.07230v1 2022-01-20,Algorithm for constructing customized quantized resistances in graphene $p-n$ junctions,"An algorithm is introduced for predicting quantized resistances in graphene p-n junction devices that utilize more than a single entry and exit point for electron flow. Depending on the configuration of an arbitrary number of terminals, electrical measurements yield fractional multiples of the typical quantized Hall resistance at the $\nu=2$ plateau $R_H \approx 12906 {\Omega}$ and take the form: $\frac{a}{b}R_H$. This theoretical formulation is independent of material, and applications to other material systems that exhibit quantum Hall behaviors are to be expected. Furthermore, this formulation is supported with experimental data from graphene-based devices with multiple source and drain terminals.",2201.08290v1 2022-12-08,Terahertz photoconductivity in bilayer graphene transistors: evidence for tunneling at gate-induced junctions,"Photoconductivity of novel materials is the key property of interest for design of photodetectors, optical modulators, and switches. Despite the photoconductivity of most novel 2d materials has been studied both theoretically and experimentally, the same is not true for 2d p-n junctions that are necessary blocks of most electronic devices. Here, we study the sub-terahertz photocoductivity of gapped bilayer graphene with electrically-induced p-n junctions. We find a strong positive contribution from junctions to resistance, temperature resistance coefficient and photo-resistivity at cryogenic temperatures T ~ 20 K. The contribution to these quantities from junctions exceeds strongly the bulk values at uniform channel doping even at small band gaps ~ 10 meV. We further show that positive junction photoresistance is a hallmark of interband tunneling, and not of intra-band thermionic conduction. Our results point to the possibility of creating various interband tunneling devices based on bilayer graphene, including steep-switching transistors and selective sensors.",2212.04378v1 2024-03-17,Resistive and ballistic phonon transport in $β$-Ga$_2$O$_3$,"The anisotropic thermal conductivity and the phonon mean free path (mfp) in monoclinic $\beta$-Ga$_2$O$_3$ single crystals and homoepitaxial films of several $\mu$m were determined using the 3$\omega$-method in the temperature range from 10K-300 K. The measured effective thermal conductivity of both, single crystal and homoepitaxial films are in the order of 20 W/(mK) at room temperature, below 30 K it increases with a maximum of 1000 to 2000 W/(mK) and decreases with T$^3$ below 25 K. Analysis of the phonon mfp shows a dominance of phonon-phonon-Umklapp scattering above 80 K, below which the influence of point-defect scattering is observed. Below 30 K the phonon mfp increases until it is limited by the total $\beta$-Ga$_2$O$_3$ sample size. A crossover from resistive to ballistic phonon transport is observed below 20 K and boundary effects of the total sample size become dominant. This reveals that the homoepitaxial film-substrate interface is highly phonon-transparent. The resistive and ballistic phonon transport regimes in $\beta$-Ga$_2$O$_3$ are discussed corresponding to the models of Callaway and Majumdar, respectively.",2403.11341v1 2004-05-05,Low temperature field-effect in crystalline organic material,"Molecular organic materials offer the promise of novel electronic devices but also present challenges for understanding charge transport in narrow band systems. Low temperature studies elucidate fundamental transport processes. We report the lowest temperature field effect transport results on a crystalline oligomeric organic material, rubrene. We find field effect switching with on-off ratio up to 10^7 at temperatures down to 10 K. Gated transport shows a factor of ~10 suppression of the thermal activation energy in 10-50 K range and nearly temperature independent resistivity below 10 K.",0405077v1 2022-07-22,Fabrication of highly resistive NiO thin films for nanoelectronic applications,"Thin films of the prototypical charge transfer insulator NiO appear to be a promising material for novel nanoelectronic devices. The fabrication of the material is challenging however, and mostly a p-type semiconducting phase is reported. Here, the results of a factorial experiment are presented that allow optimization of the film properties of thin films deposited using sputtering. A cluster analysis is performed, and four main types of films are found. Among them, the desired insulating phase is identified. From this material, nanoscale devices are fabricated, which demonstrate that the results carry over to relevant length scales. Initial switching results are reported.",2207.10837v1 2022-11-15,Nucleation and development of multiple cracks in thin composite fibers,"We study the nucleation and development of crack patterns in thin composite fibers under tension in this work. A fiber comprises an elastic core and an outer layer of a weaker brittle material. In recent tensile experiments on such composites, multiple cracks were observed to develop simultaneously on the outer layer. We propose here a simple one-dimensional model to predict such phenomenon. We idealize the problem as two axially loaded rods coupled by a linear interfacial condition. The latter can be regarded as an adhesive that resists slip between the two materials. One rod is modeled as a brittle material, and the other a linearly elastic material, both undergoing finite deformations.",2212.02232v1 2024-05-19,"Modes, Bounds, and Synthesis of Optimal Electromagnetic Scatterers","This paper presents an optimal synthesis of material distributions in obstacles for maximal extinction, scattering, or absorption. The material synthesis is based on an explicit construction utilizing the current distribution derived from physical bounds excited from the far-field. The bounds are expressed in radiation modes for materials restricted by their resistivity and characteristic modes for materials restricted by the contrast. The results are valid for arbitrary shapes, and analytical expressions are provided for spherical shapes.",2405.11499v1 2002-10-29,Electrical anisotropy in high-Tc granular superconductors in a magnetic field,"We propose an analytical model devoted to explain the anisotropy of the electrical resistance observed below the critical temperature in granular high-Tc superconductors submitted to a magnetic field H. Reported experimental results obtained on a YBCO sample show that the superconducting transition occurs in two stages, with a steep drop of the resistance at Tc and a subsequent, smoother decrease. In this second stage, the resistance vs. temperature curve is strongly dependent not only on the field intensity, but also on the angle between H and the macroscopic current density j. We start from the assumption that the resistance below Tc is mainly due to the weak links between grains. In the model, weak links are thought of as flat surface elements separating adjacent grains. We calculate the probability for a weak link to undergo the transition to the resistive state, as a function of the angles it makes with the external magnetic field H and the macroscopic current density j. In doing this, an important role is given to the strong non-uniformity of the local magnetic field within the specimen, due to the effect of the screening supercurrents flowing on the surface of the grains. Finally, we calculate the electrical resistance of the sample in the two cases where H is parallel and perpendicular to j, respectively. The predictions of this simple model turn out to be in reasonable agreement with reported experimental results obtained on a YBCO granular specimen.",0210648v1 2008-02-20,In-plane current-voltage characteristics and oscillatory Josephson-vortex flow resistance in La-free Bi$_{2+x}$Sr$_{2-x}$CuO$_{6+δ}$ single crystals in high magnetic fields,"We have investigated the in-plane $I(V)$ characteristics and the Josephson vortex flow resistance in high-quality La-free Bi$_{2+x}$Sr$_{2-x}$CuO$_{6+\delta}$ (Bi2201) single crystals in parallel and tilted magnetic fields at temperatures down to 40 mK. For parallel magnetic fields below the resistive upper critical field $H^{*}_{c2}$, the $I(V)$ characteristic obey a power-law with a smooth change with increasing magnetic-field of the exponent from above 5 down to 1. In contrast to the double-layer cuprate Bi2212, the observed smooth change suggests that there is no change in the mechanism of dissipation (no Kosterlitz-Thouless transition) over the range of temperatures investigated. At small angles between the applied field and the $ab$-plane, prominent current steps in the $I(V)$ characteristics and periodic oscillations of Josephson-vortex flow resistance are observed. While the current steps are periodic in the voltage at constant fields, the voltage position of the steps, together with the flux-flow voltage, increases nonlinearly with magnetic field. The $ab$-flow resistance oscillates as a function of field with a constant period over a wide range of magnetic fields and temperatures. The current steps in the $I(V)$ characteristics and the flow resistance oscillations can be linked to the motion of Josephson vortices across layers.",0802.2791v1 2009-06-01,Phase study of oscillatory resistances in microwave-irradiated- and dark- GaAs/AlGaAs devices: Indications of a new class of integral quantum Hall effect,"We report the experimental results from a dark study and a photo-excited study of the high mobility GaAs/AlGaAs system at large filling factors, $\nu$. At large-$\nu$, the dark study indicates several distinct phase relations (""Type-1"", ""Type-2"", and ""Type-3"") between the oscillatory diagonal- and Hall- resistances, as the canonical Integral Quantum Hall Effect (IQHE) is manifested in the ""Type-1"" case of approximately orthogonal diagonal- and Hall resistance- oscillations. Surprisingly, the investigation indicates quantum Hall plateaus also in the ""Type-3"" case characterized by approximately ""anti-phase"" Hall- and diagonal- resistance oscillations, suggesting a new class of IQHE. Transport studies under microwave photo-excitation exhibit radiation-induced magneto-resistance oscillations in both the diagonal, $R_{xx}$, and off-diagonal, $R_{xy}$, resistances. Further, when the radiation-induced magneto-resistance oscillations extend into the quantum Hall regime, there occurs a radiation-induced non-monotonic variation in the amplitude of Shubnikov-de Haas (SdH) oscillations in $R_{xx}$ \textit{vs}. B, and a non-monotonic variation in the width of the quantum Hall plateaus in $R_{xy}$. The latter effect leads into the vanishing of IQHE at the minima of the radiation-induced $R_{xx}$ oscillations with increased photo-excitation. We reason that the mechanism which is responsible for producing the non-monotonic variation in the amplitude of SdH oscillations in $R_{xx}$ under photo-excitation is also responsible for eliminating, under photo-excitation, the novel ""Type-3"" IQHE in the high mobility specimen.",0906.0032v1 2016-10-19,Pressure induced superconductivity in Bi single crystals,"Measurements on resistivity and magnetic susceptibility have been carried out for Bi single crystals under pressures up to 10.5GPa. The temperature dependent resistivity shows a semimetallic behavior at ambient and low pressures (below about 1.6GPa). This is followed by an upturn of resistivity in low temperature region when the pressure is increased, which is explained as a semiconductor behavior. This feature gradually gets enhanced up to a pressure of about 2.52GPa. Then a non-monotonic temperature dependent resistivity appears upon further increasing pressure, which is accompanied by a strong suppression to the low temperature resistivity upturn. Simultaneously, a superconducting transition occurs at about 3.92K under a pressure of about 2.63GPa. With further increasing pressure, a second superconducting transition emerges at about 7K under about 2.8GPa. For these two superconducting states, the superconductivity induced magnetic screening volumes are quite large. As the pressure further increased to 8.1GPa, we observe the third superconducting transition at about 8.2K. The resistivity measurements under magnetic field allow us to determine the upper critical fields $\mu_0 H_{c2}$ of the superconducting phases. The upper critical field for the phase with $T_c=3.92$K is extremely low. Based on the Werthamer-Helfand-Hohenberg (WHH) theory, the estimated value of $\mu_0 H_{c2}$ for this phase is about 0.103T. While the upper critical field for the phase with $T_c$=7K is very high with a value of about 4.56T. Finally, we present a pressure dependent phase diagram of Bi single crystals. Our results reveal the interesting and rich physics in bismuth single crystals under high pressure.",1610.06062v1 2021-01-14,Effects of resistivity on standing shocks in low angular momentum flows around black holes,"We study two dimensional low angular momentum flow around the black hole using the resistive magnetohydrodynamic module of PLUTO code. Simulations have been performed for the flows with parameters of specific angular momentum, specific energy, and magnetic field which may be expected for the flow around Sgr A*. For flows with lower resistivity $\eta=10^{-6}$ and $0.01$, the luminosity and the shock location on the equator vary quasi-periodically. The power density spectra of luminosity variation show the peak frequencies which correspond to the periods of $5 \times 10^5$, $1.4 \times 10^5$, and $5 \times 10^4$ seconds, respectively. These quasi-periodic oscillations (QPOs) occur due to the interaction between the outer oscillating standing shock and the inner weak shocks occurring at the innermost hot blob. While for cases with higher resistivity $\eta=0.1$ and 1.0, the high resistivity considerably suppresses the magnetic activity such as the MHD turbulence and the flows tend to be steady and symmetric to the equator. The steady standing shock is formed more outward compared with the hydrodynamical flow. The low angular momentum flow model with the above flow parameters and with low resistivity has a possibility for the explanation of the long-term flares with $\sim$ one per day and $\sim 5 - 10$ days of Sgr A* in the latest observations by Chandra, Swift, and XMM-Newton monitoring of Sgr A*.",2101.05474v2 2014-06-19,AC loss and coupling currents in YBCO coated conductors with varying number of filaments,"Striation of HTS coated conductors (CCs) as a way to reduce their magnetization AC losses has been the subject of intense research in the past years by several groups. While the principle of this approach is well understood, its practical application on commercial material to be used in power application is still far to be implemented due to manufacturing and technological constraints. Recent advances in tape quality and striation technology are now enabling systematic investigations of the influence of the number of filaments on AC loss reduction with a consistency that was not available in the past. In this work we demonstrate the technological feasibility of reducing the magnetization losses of commercially available CC by striating them into a high number of filaments (up to 120). The loss reduction exceeds one order of magnitude and does not come at the expense of current-carrying capability: samples with 10 and 20 filaments are unaffected by the striation process, while samples with 80 and 120 filaments still retain 80 and 70% of the current-carrying potential, respectively. We also investigate the transverse resistivity in order to understand the paths followed by the coupling currents: we found that the coupling current prevalently flows in the metallic substrate, rather than in and out of the filaments. Finally, we use oxidation as a method to reduce the coupling currents and losses. The contribution of this work is three-fold: 1) It describes the know-how to produce a large number of high quality striations in commercially available CCs, greatly reducing their losses without extensively degrading their transport properties; 2) It provides a comprehensive characterization of said samples (e.g. measurements in a wide frequency range, transverse resistance profiles, influence of oxidation on DC and AC behavior); 3) It provides new insight on the patterns of the coupling currents.",1406.4990v2 2017-09-21,Electrical properties of single crystal Yttrium Iron Garnet ultra-thin films at high temperatures,"We report a study on the electrical properties of 19 nm thick Yttrium Iron Garnet (YIG) films grown by liquid phase epitaxy. The electrical conductivity and Hall coefficient are measured in the high temperature range [300,400]~K using a Van der Pauw four-point probe technique. We find that the electrical resistivity decreases exponentially with increasing temperature following an activated behavior corresponding to a band-gap of $E_g\approx 2$ eV, indicating that epitaxial YIG ultra-thin films behave as large gap semiconductor, and not as electrical insulator. The resistivity drops to about $5\times 10^3$~$\Omega \cdot \text{cm}$ at $T=400$ K. We also infer the Hall mobility, which is found to be positive ($p$-type) at 5 cm$^2$/(V$\cdot$sec) and about independent of temperature. We discuss the consequence for non-local transport experiments performed on YIG at room temperature. These electrical properties are responsible for an offset voltage (independent of the in-plane field direction) whose amplitude, odd in current, grows exponentially with current due to Joule heating. These electrical properties also induce a sensitivity to the perpendicular component of the magnetic field through the Hall effect. In our lateral device, a thermoelectric offset voltage is produced by a temperature gradient along the wire direction proportional to the perpendicular component of the magnetic field (Righi-Leduc effects).",1709.07207v1 2020-04-01,Perovskite-type cobalt oxide at the multiferroic Co/Pb Zr$_{0.2}$Ti$_{0.8}$O$_{3}$ interface,"Magnetic Tunnel Junctions whose basic element consists of two ferromagnetic electrodes separated by an insulating non-magnetic barrier have become intensely studied and used in non-volatile spintronic devices. Since ballistic tunnel of spin-polarized electrons sensitively depends on the chemical composition and the atomic geometry of the lead/barrier interfaces their proper design is a key issue for achieving the required functionality of the devices such as e.g. a high tunnel magneto resistance. An important leap in the development of novel spintronic devices is to replace the insulating barrier by a ferroelectric which adds new additional functionality induced by the polarization direction in the barrier giving rise to the tunnel electro resistance (TER). The multiferroic tunnel junction Co/PbZr$_{0.2}$Ti$_{0.8}$O$_{3}$/La$_{2/3}$Sr$_{1/3}$MnO$_3$ (Co/PZT/LSMO) represents an archetype system for which - despite intense studies - no consensus exists for the interface geometry and their effect on transport properties. Here we provide the first analysis of the Co/PZT interface at the atomic scale using complementary techniques, namely x-ray diffraction and extended x-ray absorption fine structure in combination with x-ray magnetic circular dichroism and ab-initio calculations. The Co/PZT interface consists of one perovskite-type cobalt oxide unit cell [CoO$_{2}$/CoO/Ti(Zr)O$_{2}$] on which a locally ordered cobalt film grows. Magnetic moments (m) of cobalt lie in the range between m=2.3 and m=2.7$\mu_{B}$, while for the interfacial titanium atoms they are small (m=+0.005 $\mu_{B}$) and parallel to cobalt which is attributed to the presence of the cobalt-oxide interface layers. These insights into the atomistic relation between interface and magnetic properties is expected to pave the way for future high TER devices.",2004.00489v1 2020-05-26,"Influence of Different Surface Morphologies on the Performance of High Voltage, Low Resistance Diamond Schottky Diodes","Vertical diamond Schottky diodes with blocking voltages $V_{\text{BD}} > 2.4 \text{ kV}$ and on-resistances $R_{\text{On}} < 400 \text{ m}\Omega \text{cm}^{2}$ were fabricated on homoepitaxially grown diamond layers with different surface morphologies. The morphology (smooth as-grown, hillock-rich, polished) influences the Schottky barrier, the carrier transport properties, and consequently the device performance. The smooth as-grown sample exhibited a low reverse current density $J_{\text{Rev}} < 10^{-4} \text{ A}/\text{cm}^{2}$ for reverse voltages up to $2.2 \text{ kV}$. The hillock-rich sample blocked similar voltages with a slight increase in the reverse current density ($J_{\text{Rev}} < 10^{-3} \text{ A}/\text{cm}^{2}$). The calculated 1D-breakdown field, however, was reduced by $30 \text{ } \%$, indicating a field enhancement induced by the inhomogeneous surface. The polished sample demonstrated a similar breakdown voltage and reverse current density as the smooth as-grown sample, suggesting that a polished surface can be suitable for device fabrication. However, a statistical analysis of several diodes of each sample showed the importance of the substrate quality: A high density of defects both reduces the feasible device area and increases the reverse current density. In forward direction, the hillock-rich sample exhibited a secondary Schottky barrier, which could be fitted with a modified thermionic emission model employing the Lambert W-function. Both polished and smooth sample showed nearly ideal thermionic emission with ideality factors $1.08$ and $1.03$, respectively. Compared with literature, all three diodes exhibit an improved Baliga Figure of Merit for diamond Schottky diodes with $V_{\text{BD}} > 2 \text{ kV}$.",2005.12591v1 2023-11-21,Evidence of filamentary superconductivity in pressurized La3Ni2O7,"Recently, the signatures of superconductivity near 80 K have been discovered in the single crystal of La3Ni2O7 under pressure, which makes it a new candidate of the high-temperature superconductors dominated by 3d transition elements after the cuprate and iron-pnictide superconductors, and thus has attracted significant attention. However, the superconductivity, characterized by the zero resistance and the Meissner effect, is anomalously irreproducible in the compressed La3Ni2O7. In this study, we report the experimental results obtained through highly sensitive modulated ac susceptibility measurements, which reveal that the maximum superconducting volume fraction in the La3Ni2O7 sample is only approximately 1% (employing superconducting element vanadium as a reference). In tandem with our observation of the zero-resistance state only in some of the samples, we suggest that the superconductivity in this nickelate is filamentary-like. In combination of our scanning transmission electron microscopy (STEM) investigations, we propose that the filamentary superconductivity most likely emerges at the interface between the La3Ni2O7 and La4Ni3O10 phases. Further, the connection of the oxygen vacancy in La3Ni2O7 with the presence of superconductivity and superconducting transition temperature (Tc) has been established, through which the upper and lower bounds of the oxygen content for the presence of superconductivity were determined to be 6.89 and 7.35, respectively. Our results not only provide new insights into understanding the puzzling issues in this material, but also highlight a new route for exploring new high-Tc nickelate superconductors with a higher superconducting volume fraction, as well as pose a new challenge in comprehending the complex nature of this filamentary superconductivity.",2311.12361v2 2024-03-01,Electrochemical Evaluation of Mg and a Mg-Al 5%Zn Metal Rich Primers for Protection of Al-Zn-Mg-Cu Alloy in NaCl,"High purity magnesium and a Mg-Al 5wt% Zn metal rich primer (MRP) were compared for their ability to suppress intergranular corrosion (IGC) and intergranular stress corrosion cracking (IG-SCC) in peak aged AA 7075-T651 by sacrificial anode-based cathodic prevention. Tests were conducted in 0.6 M NaCl solution under full immersion. These evaluations considered the ability of the primer to attain an intermediate negative open circuit potential (OCP) such that the galvanic couple potential with bare aluminum alloy (AA) 7075-T651 resided below a range of potentials where IGC is prevalent. The ability of the primer to achieve an OCP negative enough that the AA 7075-T651 could be protected by sacrificial anode-based cathodic prevention and the ability to sustain this function over time were evaluated as a first step by utilizing a NaCl solution. The primers consisted of epoxy resins embedded with either (1) Mg flake pigments (MgRP) or (2) Mg flake pigments and spherical Al-5 wt.% Zn together as a composite (MgAlRP). MgRP was an effective coating for cathodic protection but dispensed less anodic charge than the composite MgAlRP. Cross-sectional analysis demonstrated that some Mg flakes dissolved while uniform surface oxidation occurred on the remaining Mg flakes which led to impaired activation. The composite MgAlRP maintained a suitably negative OCP over time, remained activated, dispensed high anodic charge, and remained an anode in zero resistance ammeter testing. Chemical stability modeling and zero resistance ammeter testing suggest that Mg corrosion elevates the pH which dissolved aluminum oxides and hydroxide thereby activates the Al-5wt.% Zn pigments, thereby providing a primary (i.e. Mg corrosion) and secondary process to enable superior (activation of Al-5wt%Zn) sacrificial anode-based cathodic protection.",2403.00610v1 2007-09-14,High pressure study on the strong-coupling superconductivity in non-centrosymmetric compound CeIrSi_3,"We have carried out high pressure experiment on the pressure-induced superconductor CeIrSi$_3$ without inversion center. The electrical resistivity and ac heat capacity were measured in the same run for the same sample. The critical pressure of the antiferromagnetic state was determined to be $P_{\rm c}$ = 2.25 GPa. The heat capacity $C_{\rm ac}$ shows both antiferromagnetic and superconducting transitions at pressures close to $P_{\rm c}$. The superconducting transition temperature $T_{\rm sc}$ shows a maximum value of 1.6 K around $2.5-2.7$ GPa. At 2.58 GPa, a large heat capacity anomaly was observed at $T_{\rm sc}$ = 1.59 K. The jump of the heat capacity in the form of ${\Delta}{C_{\rm ac}}/C_{\rm ac}(T_{\rm sc})$ is 5.7 $\pm$ 0.1. This is the largest value observed among all superconductors studied previously, suggesting the strong-coupling superconductivity in CeIrSi$_3$. The large magnitude and anisotropy of the upper critical field $B_{\rm c2}$ at 2.65 GPa is discussed from view points of the strong-coupling superconductivity and the reduced paramagnetic effect in the non-centrosymmetric superconductor. Above $P_{\rm c}$, the electrical resistivity shows the anomalous $T$-linear dependence in the wide temperature region from $T_{\rm sc}$ to 30 K, which is different from the Fermi liquid theory. Meanwhile, the heat capacity $C_{\rm ac}/T$ shows a simple temperature dependence in the normal state above $T_{\rm sc}$. These features do not seem to be explained simply by the spin fluctuation theory. The electronic specific heat coefficient at $T_{\rm sc}$ is approximately unchanged as a function of pressure, even at $P_{\rm c}$.",0709.2199v1 2016-06-09,Ternary borides Nb$_7$Fe$_3$B$_8$ and Ta$_7$Fe$_3$B$_8$ with Kagome-type iron framework,"Two new ternary borides $TM$$_7$Fe$_3$B$_8$ ($TM$ = Nb, Ta) were synthesized by high-temperature thermal treatment of samples obtained by arc-melting. This new type of structure with space group $P$6/$mmm$, comprises $TM$ slabs containing isolated planar hexagonal [B$_6$] rings and iron centered $TM$ columns in a Kagome type of arrangement. Chemical bonding analysis in Nb$_7$Fe$_3$B$_8$ by means of the electron localizability approach reveals two-center interactions forming the Kagome net of Fe and embedded B, while weaker multicenter bonding present between this net and Nb atoms. Magnetic susceptibility measurements reveal antiferromagnetic order below $T_N$ = 240 K for Nb$_7$Fe$_3$B$_8$ and $T_N$ =265 K for Ta$_7$Fe$_3$B$_8$. Small remnant magnetization below 0.01 $\mu_B$/f.u. is observed in the antiferromagnetic state. The bulk nature of the magnetic transitions was confirmed by the hyperfine splitting of the M\""o{\ss}bauer spectra, the sizable anomalies in the specific heat capacity, and the kinks in the resistivity curves. The high-field paramagnetic susceptibilities fitted by the Curie-Weiss law show effective paramagnetic moments $\mu_{eff}$ about 3.1 $\mu_B$/Fe in both compounds. The temperature dependence of the electrical resistivity also reveals metallic character of both compounds. Density functional calculations corroborate the metallic behaviour of both compounds and demonstrate the formation of a sizable local magnetic moment on the Fe-sites. They indicate the presence of both antiferro- and ferromagnetic interactions.",1606.03123v1 2020-01-24,Quantum transport in topological surface states of Bi$_2$Te$_3$ nanoribbons,"Quasi-1D nanowires of topological insulators are emerging candidate structures in superconductor hybrid architectures for the realization of Majorana fermion based quantum computation schemes. It is however technically difficult to both fabricate as well as identify the 1D limit of topological insulator nanowires. Here, we investigated selectively-grown Bi$_2$Te$_3$ topological insulator nanoribbons and nano Hall bars at cryogenic temperatures for their topological properties. The Hall bars are defined in deep-etched Si$_3$N$_4$/SiO$_2$ nano-trenches on a silicon (111) substrate followed by a selective area growth process via molecular beam epitaxy. The selective area growth is beneficial to the device quality, as no subsequent fabrication needs to be performed to shape the nanoribbons. Transmission line measurements are performed to evaluate contact resistances of Ti/Au contacts applied as well as the specific resistance of the Bi$_2$Te$_3$ binary topological insulator. In the diffusive transport regime of these unintentionally $n$-doped Bi$_2$Te$_3$ topological insulator nano Hall bars, we identify distinguishable electron trajectories by analyzing angle-dependent universal conductance fluctuation spectra. When the sample is tilted from a perpendicular to a parallel magnetic field orientation, these high frequent universal conductance fluctuations merge with low frequent Aharonov-Bohm type oscillations originating from the topologically protected surface states encircling the nanoribbon cross section. For 500 nm wide Hall bars we also identify low frequent Shubnikov-de Haas oscillations in the perpendicular field orientation, that reveal a topological high-mobility 2D transport channel, partially decoupled from the bulk of the material.",2001.09028v1 2020-06-01,"PrVO$_4$ under High Pressure: Effects on Structural, Optical and Electrical Properties","In pursue of a systematic characterization of rare-earth vanadates under compression, in this work we present a multifaceted study of the phase behavior of zircon-type orthovanadate PrVO$_4$ under high pressure conditions, up until 24 GPa. We have found that PrVO$_4$ undergoes a zircon to monazite transition at around 6 GPa, confirming previous results found by Raman experiments. A second transition takes place above 14 GPa, to a BaWO$_4$-I--type structure. The zircon to monazite structural sequence is an irreversible first-order transition, accompanied by a volume collapse of about 9.6%. Monazite phase is thus a metastable polymorph of PrVO$_4$. The monazite-BaWO$_4$-II transition is found to be reversible instead and occurs with a similar volume change. Here we report and discuss the axial and bulk compressibility of all phases. We also compare our results with those for other rare-earth orthovanadates. Finally, by means of optical-absorption experiments and resistivity measurements we determined the effect of pressure on the electronic properties of PrVO$_4$. We found that the zircon-monazite transition produces a collapse of the band gap and an abrupt decrease of the resistivity. The physical reasons for this behavior are discussed. Density-functional-theory simulations support our conclusions.",2006.01299v2 2024-04-04,"Electronic transport, metal-insulator transition, and Wigner crystallization in transition metal dichalcogenide monolayers","Two recent electronic transport experiments from Columbia University and Harvard University have reported record high mobility and low channel densities in transition metal dichalcogenide (TMD) WSe$_2$ monolayers [J. Pack, et al., arXiv:2310.19782; A. Y. Joe, et al., Phys. Rev. Lett. 132, 056303 (2024)]. A two-dimensional (2D) metal-insulator transition (MIT) is demonstrated in the Columbia sample at low densities, a regime where the formation of a Wigner crystal (WC) is theoretically anticipated in the absence of disorder. We employ the finite-temperature Boltzmann theory to understand the low-temperature transport properties of monolayer TMDs, taking into account realistic disorder scattering. We analyze the experimental results, focusing on the 2D MIT behavior and the influence of temperature and density on mobility and resistivity in the metallic phase. We provide a discussion of the nontrivial carrier density dependence of our transport results. Our analysis elucidates the linear-in-$T$ resistivity in the metallic phase, attributing it to Friedel oscillations associated with screened charged impurities. Furthermore, we explore whether Coulomb disorder could lead to the MIT through either a quantum Anderson localization transition or a classical percolation transition. Our theoretical estimates of the disorder-induced MIT critical densities, although smaller, are within a factor of ~2 of the experimental critical density. We examine the exceptionally high melting temperature ~10 K of WCs observed experimentally in the MoSe$_2$ systems at low density, an order of magnitude larger than the pristine melting temperature. This suggests that the observed 2D low-density MIT behavior is likely a result of the complex interplay between disorder effects and interaction-driven WC physics, offering a comprehensive understanding of the low-temperature transport phenomena in TMD monolayers.",2404.03488v1 2005-06-08,X-ray Diagnostics of Grain Depletion in Matter Accreting onto T Tauri Stars,"Recent analysis of high resolution Chandra X-ray spectra has shown that the Ne/O abundance ratio is remarkably constant in stellar coronae. Based on this result, we point out the utility of the Ne/O ratio as a discriminant for accretion-related X-rays from T Tauri stars, and for probing the measure of grain-depletion of the accreting material in the inner disk. We apply the Ne/O diagnostic to the classical T Tauri stars BP Tau and TW Hya--the two stars found to date whose X-ray emission appears to originate, at least in part, from accretion activity. We show that TW Hya appears to be accreting material which is significantly depleted in O relative to Ne. In constrast, BP Tau has an Ne/O abundance ratio consistent with that observed for post-T Tauri stars. We interpret this result in terms of the different ages and evolutionary states of the circumstellar disks of these stars. In the young BP Tau disk (age 0.6 Myr) dust is still present near the disk corotation radius and can be ionized and accreted, re-releasing elements depleted onto grains. In the more evolved TW Hya disk (age 10 Myr), evidence points to ongoing coagulation of grains into much larger bodies, and possibly planets, that can resist the drag of inward-migrating gas, and accreting gas is consequently depleted of grain-forming elements.",0506185v1 2003-02-13,"Electronic phase separation in the rare earth manganates, (La1-xLnx)0.7Ca0.3MnO3 (Ln = Nd, Gd and Y)","All the three series of manganates showsaturation magnetization characteristic of ferromagnetism, with the ferromagnetic Tc decreasing with increasing in x up to a critical value of x, xc (xc = 0.6, 0.3, 0.2 respectively for Nd, Gd, Y). For x > xc, the magnetic moments are considerably smaller showing a small increase around TM, the value of TM decreasing slightly with increase in x or decrease in < rA >. The ferromagnetic compositions (x xc) show insulator-metal (IM) transitions, while the compositions with x > xc are insulating. The magnetic and electrical resistivity behavior of these manganates is consistent with the occurrence of phase separation in the compositions around xc, corresponding to a critical average radius of the A-site cation, < rAc >, of 1.18 A. Both Tc and TIM increase linearly when < rA > > < rAc > or x xc as expected of a homogenous ferromagnetic phase. Both Tc and TM decrease linearly with the A-site cation size disorder at the A-site as measured by the variance s2. Thus, an increase in s2 favors the insulating AFM state. Percolative conduction is observed in the compositions with < rA > > < rAc >. Electron transport properties in the insulating regime for x > xc conforms to the variable range hopping mechanism. More interestingly, when x > xc, the real part of dielectric constant (e') reaches a high value (104-106) at ordinary temperatures dropping to a very small (~500) value below a certain temperature, the value of which decreases with decreasing frequency.",0302268v1 2003-03-21,"Independent Electronic and Magnetic Doping in (Ga,Mn)As Based Digital Ferromagnetic Heterostructures","Ferromagnetic semiconductors promise the extension of metal-based spintronics into a material system that combines widely tunable electronic, optical, and magnetic properties. Here, we take steps towards realizing that promise by achieving independent control of electronic doping in the ferromagnetic semiconductor (Ga,Mn)As. Samples are comprised of superlattices of 0.5 monolayer (ML) MnAs alternating with 20 ML GaAs and are grown by low temperature (230 C) atomic layer epitaxy (ALE). This allows for the reduction of excess As incorporation and hence the number of charge-compensating As-related defects. We grow a series of samples with either Be or Si doping in the GaAs spacers (p- and n-type dopants, respectively), and verify their structural quality by in situ reflection high-energy electron diffraction (RHEED) and ex situ x-ray diffraction. Magnetization measurements reveal ferromagnetic behavior over the entire doping range, and show no sign of MnAs precipitates. Finally, magneto-transport shows the giant planar Hall effect and strong (20%) resistance fluctuations that may be related to domain wall motion.",0303461v1 2006-02-26,Physical properties and magnetic structure of TbRhIn5 intermetallic compound,"In this work we report the physical properties of the new intermetallic compound TbRhIn5 investigated by means of temperature dependent magnetic susceptibility, electrical resistivity, heat-capacity and resonant x-ray magnetic diffraction experiments. TbRhIn5 is an intermetallic compound that orders antiferromagnetically at TN = 45.5 K, the highest ordering temperature among the existing RRhIn5 (1-1-5, R = rare earth) materials. This result is in contrast to what is expected from a de Gennes scaling along the RRhIn5 series. The X-ray resonant diffraction data below TN reveal a commensurate antiferromagnetic (AFM) structure with a propagation vector (1/2 0 1/2) and the Tb moments oriented along the c-axis. Strong (over two order of magnitude) dipolar enhancements of the magnetic Bragg peaks were observed at both Tb absorption edges LII and LIII, indicating a fairly high polarization of the Tb 5d levels. Using a mean field model including an isotropic first-neighbors exchange interaction J(R-R) and the tetragonal crystalline electrical field (CEF), we were able to fit our experimental data and to explain the direction of the ordered Tb-moments and the enhanced TN of this compound. The evolution of the magnetic properties along the RRhIn5 series and its relation to CEF effects for a given rare-earth is discussed.",0602612v1 2006-06-28,Dielectric anomaly at the orbital order-disorder transition in LaMnO_(3+delta),"We report a novel dielectric anomaly around the Jahn-Teller orbital order-disorder transition temperature T_JT in LaMnO_(3+delta). The transition has been characterized by resistivity (rho)versus temperature (T), calorimetry, and temperature-dependent X-ray diffraction studies. Measurements of complex dielectric permittivity epsilon* (= epsilon'-i.epsilon'') over a low-frequency range (1 Hz - 10 MHz)across T_JT reveal a distinct anomaly. This observation, and the reported relatively high static dielectric constant at T = 0 (epsilon0 \~18-20), possibly indicate that the orbital order gives rise to intrinsic polarization that undergoes transition at T_JT. The frequency dispersion of the dielectric response at any given temperature, however, reveals that the dielectric response consists of Maxwell-Wagner component, due to interfaces, within such a low frequency range. The T_JT and the nature of the anomaly in epsilon'(omega,T), epsilon''(omega,T) at T_JT, of course, vary - from a sharp upward feature to a smeared plateau and then a downward trend - depending on the Mn^4+ concentration of the sample. The observation of an intrinsic dielectric response due to long-range orbital order in LaMnO_3 - where no ferroelectric order is possible due to the absence of off-centre distortion in MnO_6 octahedra - may throw a new light onto these classes of materials vis-a-vis multiferroic materials.",0606731v1 2003-10-07,Role of Oxygen and Carbon Impurities in the Radiation Resistance of Silicon Detectors,"The influence of oxygen and carbon impurities on the concentrations of defects in silicon for detector uses, in complex fields of radiation (proton cosmic field at low orbits around the Earth, at Large Hadron Collider and at the next generation of accelerators as Super-LHC) is investigated in the frame of the quantitative model developed previously by the authors. The generation rate of primary defects is calculated starting from the projectile - silicon interaction and from recoil energy redistribution in the lattice. The mechanisms of formation of complex defects are explicitly analysed. Vacancy-interstitial annihilation, interstitial and vacancy migration to sinks, divacancy, vacancy and interstitial impurity complex formation and decomposition are considered. Oxygen and carbon impurities present in silicon could monitor the concentration of all stable defects, due to their interaction with vacancies and interstitials. Their role in the mechanisms of formation and decomposition of the following stable defects: VP, VO, V_2, V_2O, C_i, C_iO_i and C_iC_s is studied. The model predictions could be a useful clue in obtaining harder materials for detectors at the new generation of accelerators, for space missions or for industrial applications.",0310032v1 2009-01-22,Signal height in silicon pixel detectors irradiated with pions and protons,"Pixel detectors are used in the innermost part of multi purpose experiments at the Large Hadron Collider (LHC) and are therefore exposed to the highest fluences of ionising radiation, which in this part of the detectors consists mainly of charged pions. The radiation hardness of the detectors has thoroughly been tested up to the fluences expected at the LHC. In case of an LHC upgrade the fluence will be much higher and it is not yet clear up to which radii the present pixel technology can be used. In order to establish such a limit, pixel sensors of the size of one CMS pixel readout chip (PSI46V2.1) have been bump bonded and irradiated with positive pions up to 6E14 Neq/cm^2 at PSI and with protons up to 5E15 Neq/cm^2. The sensors were taken from production wafers of the CMS barrel pixel detector. They use n-type DOFZ material with a resistance of about 3.7kOhm cm and an n-side read out. As the performance of silicon sensors is limited by trapping, the response to a Sr-90 source was investigated. The highly energetic beta-particles represent a good approximation to minimum ionising particles. The bias dependence of the signal for a wide range of fluences will be presented.",0901.3422v1 2012-04-17,Beta-Ag2Te: A topological insulator with strong anisotropy,"We present evidence of topological surface states in beta-Ag2Te through first-principles calculations and periodic quantum interference effect in single crystalline nanoribbon. Our first-principles calculations show that beta-Ag2Te is a topological insulator with a gapless Dirac cone with strong anisotropy. To experimentally probe the topological surface state, we synthesized high quality beta-Ag2Te nanoribbons and performed electron transport measurements. The coexistence of pronounced Aharonov-Bohm oscillations and weak Altshuler-Aronov-Spivak oscillations clearly demonstrates coherent electron transport around the perimeter of beta-Ag2Te nanoribbon and therefore the existence of metallic surface states, which is further supported by the temperature dependence of resistivity for beta-Ag2Te nanoribbons with different cross section areas. Highly anisotropic topological surface state of beta-Ag2Te suggests that the material is a promising material for fundamental study and future spintronic devices.",1204.3816v6 2012-09-16,Glass-like recovery of antiferromagnetic spin ordering and dimensional crossover in a photo-excited manganite Pr$_{0.7}$Ca$_{0.3}$MnO$_3$,"Electronic orderings of charges, orbitals and spins are observed in many strongly correlated electron materials, and revealing their dynamics is a critical step toward understanding the underlying physics of important emergent phenomena. Here we use time-resolved resonant soft x-ray scattering spectroscopy to probe the dynamics of antiferromagnetic spin ordering in the manganite Pr$_{0.7}$Ca$_{0.3}$MnO$_3$ following ultrafast photo-exitation. Our studies reveal a glass-like recovery of the spin ordering and a crossover in the dimensionality of the restoring interaction from quasi-1D at low pump fluence to 3D at high pump fluence. This behavior arises from the metastable state created by photo-excitation, a state characterized by spin disordered metallic droplets within the larger charge- and spin-ordered insulating domains. Comparison with time-resolved resistivity measurements suggests that the collapse of spin ordering is correlated with the insulator-to-metal transition, but the recovery of the insulating phase does not depend on the re-establishment of the spin ordering.",1209.3452v2 2013-05-30,Kelvin Probe Microscopy and Electronic Transport Measurements in Reduced Graphene Oxide Chemical Sensors,"Reduced Graphene Oxide (RGO) is an electronically hybrid material that displays remarkable chemical sensing properties. Here, we present a quantitative analysis of the chemical gating effects in RGO-based chemical sensors. The gas sensing devices are patterned in a field-effect transistor geometry, by dielectrophoretic assembly of RGO platelets between gold electrodes deposited on SiO2/Si substrates. We show that these sensors display highly selective and reversible responses to the measured analytes, as well as fast response and recovery times (tens of seconds). We use combined electronic transport/Kelvin Probe Microscopy measurements to quantify the amount of charge transferred to RGO due to chemical doping when the device is exposed to electron-acceptor (acetone) and electron-donor (ammonia) analytes. We demonstrate that this method allows us to obtain high-resolution maps of the surface potential and local charge distribution both before and after chemical doping, to identify local gate-susceptible areas on the RGO surface, and to directly extract the contact resistance between the RGO and the metallic electrodes. The method presented is general, suggesting that these results have important implications for building graphene and other nanomaterial-based chemical sensors.",1305.7222v1 2014-04-02,Direct observation of the leakage current in epitaxial diamond Schottky barrier devices by conductive-probe atomic force microscopy and Raman imaging,"The origin of the high leakage current measured in several vertical-type diamond Schottky devices is conjointly investigated by conducting probe atomic force microscopy (CP-AFM) and confocal micro-Raman/Photoluminescence (PL) imaging analysis. Local areas characterized by a strong decrease of the local resistance (5-6 orders of magnitude drop) with respect to their close surrounding have been identified in several different regions of the sample surface. The same local areas, also referenced as electrical hot-spots, reveal a slightly constrained diamond lattice and three dominant Raman bands in the low-wavenumber region (590, 914 and 1040 cm-1). These latter bands are usually assigned to the vibrational modes involving boron impurities and its possible complexes that can electrically act as traps for charge carriers. Local current-voltage measurements performed at the hot-spots point out a trap-filled-limited (TFL) current as the main conduction mechanism favoring the leakage current in the Schottky devices.",1404.0472v2 2014-09-20,Crystallization characteristics and chemical bonding properties of nickel carbide thin film nanocomposites,"The crystal structure and chemical bonding of magnetron-sputtering deposited nickel carbide Ni$_{1-x}$C$_{x}$ (0.05$\leq$x$\leq$0.62) thin films have been investigated by high-resolution X-ray diffraction, transmission electron microscopy, X-ray photoelectron spectroscopy, Raman spectroscopy, and soft X-ray absorption spectroscopy. By using X-ray as well as electron diffraction, we found carbon-containing hcp-Ni (hcp-NiC$_{y}$ phase), instead of the expected rhombohedral-Ni$_{3}$C. At low carbon content (4.9 at\%) the thin film consists of hcp-NiC$_{y}$ nanocrystallites mixed with a smaller amount of fcc-NiC$_{x}$. The average grain size is about 10-20 nm. With the increase of carbon content to 16.3 at\%, the film contains single-phase hcp-NiC$_{y}$ nanocrystallites with expanded lattice parameters. With further increase of carbon content to 38 at\%, and 62 at\%, the films transform to X-ray amorphous materials with hcp-NiC$_{y}$ and fcc-NiC$_{x }$ nanodomain structures in an amorphous carbon-rich matrix. Raman spectra of carbon indicate dominant $sp^{2}$ hybridization, consistent with photoelectron spectra that show a decreasing amount of C-Ni phase with increasing carbon content. The Ni $3d$ - C $2p$ hybridization in the hexagonal structure gives rise to the salient double-peak structure in Ni $2p$ soft X-ray absorption spectra at 16.3 at\% that changes with carbon content. We also show that the resistivity is not only governed by the amount of carbon, but increases by more than a factor of two when the samples transform from crystalline to amorphous.",1409.5912v1 2015-03-04,Signature of strong spin-orbital coupling in the large non-saturating magnetoresistance material WTe2,"We report the detailed electronic structure of WTe$_2$ by high resolution angle-resolved photoemission spectroscopy. Unlike the simple one electron plus one hole pocket type of Fermi surface topology reported before, we resolved a rather complicated Fermi surface of WTe$_2$. Specifically, there are totally nine Fermi pockets, including one hole pocket at the Brillouin zone center $\Gamma$, and two hole pockets and two electron pockets on each side of $\Gamma$ along the $\Gamma$-$X$ direction. Remarkably, we have observed circular dichroism in our photoemission spectra, which suggests that the orbital angular momentum exhibits a rich texture at various sections of the Fermi surface. As reported previously for topological insulators and Rashiba systems, such a circular dichroism is a signature for spin-orbital coupling (SOC). This is further confirmed by our density functional theory calculations, where the spin texture is qualitatively reproduced as the conjugate consequence of SOC. Since the backscattering processes are directly involved with the resistivity, our data suggest that the SOC and the related spin and orbital angular momentum textures may be considered in the understanding of the anomalous magnetoresistance of WTe$_2$.",1503.01422v1 2015-11-03,Two-dimensional epitaxial superconductor-semiconductor heterostructures: A platform for topological superconducting networks,"Progress in the emergent field of topological superconductivity relies on synthesis of new material combinations, combining superconductivity, low density, and spin-orbit coupling (SOC). For example, theory [1-4] indicates that the interface between a one-dimensional (1D) semiconductor (Sm) with strong SOC and a superconductor (S) hosts Majorana modes with nontrivial topological properties [5-8]. Recently, epitaxial growth of Al on InAs nanowires was shown to yield a high quality S-Sm system with uniformly transparent interfaces [9] and a hard induced gap, indicted by strongly suppressed sub gap tunneling conductance [10]. Here we report the realization of a two-dimensional (2D) InAs/InGaAs heterostructure with epitaxial Al, yielding a planar S-Sm system with structural and transport characteristics as good as the epitaxial wires. The realization of 2D epitaxial S-Sm systems represent a significant advance over wires, allowing extended networks via top-down processing. Among numerous potential applications, this new material system can serve as a platform for complex networks of topological superconductors with gate-controlled Majorana zero modes [1-4]. We demonstrate gateable Josephson junctions and a highly transparent 2D S-Sm interface based on the product of excess current and normal state resistance.",1511.01127v2 2015-11-08,Real-time Stress Measurements in Germanium Thin Film Electrodes during Electrochemical Lithiation/delithiation Cycling,"An in situ study of stress evolution and mechanical behavior of germanium as a lithium-ion battery electrode material is presented. Thin films of germanium are cycled in a half-cell configuration with lithium metal foil as counter/reference electrode, with 1M LiPF6 in ethylene carbonate, diethyl carbonate, dimethyl carbonate solution (1:1:1, wt. %) as electrolyte. Real-time stress evolution in the germanium thin-film electrodes during electrochemical lithiation/delithiation is measured by monitoring the substrate curvature using the multi-beam optical sensing method. Upon lithiation a-Ge undergoes extensive plastic deformation, with a peak compressive stress reaching as high as -0.76 +/- 0.05 GPa (mean +/- standard deviation). The compressive stress decreases with lithium concentration reaching a value of approximately -0.3 GPa at the end of lithiation. Upon delithiation the stress quickly became tensile and follows a trend that mirrors the behavior on compressive side; the average peak tensile stress of the lithiated Ge samples was approximately 0.83 GPa. The peak tensile stress data along with the SEM analysis was used to estimate a lower bound fracture resistance of lithiated Ge, which is approximately 5.3 J/m^2. It was also observed that the lithiated Ge is rate sensitive, i.e., stress depends on how fast or slow the charging is carried out.",1511.02442v1 2016-02-03,Full range of proximity effect probed with Superconductor/Graphene/Superconductor junctions,"The high tunability of the density of states of graphene makes it an ideal probe of quantum transport in different regimes. In particular, the supercurrent that can flow through a non-superconducting (N) material connected to two superconducting electrodes, crucially depends on the lenghth of the N relative to the superconducting coherence length. Using graphene as the N material we have investigated the full range of the superconducting proximity effect, from short to long diffusive junctions. By combining several S/graphene/S samples with different contacts and lengths, and measuring their gate-dependent critical currents ($ I_c $) and normal state resistance $ R_N $, we compare the product $eR_NI_c$ to the relevant energies, the Thouless energy in long junctions and the superconducting gap of the contacts in short junctions, over three orders of magnitude of Thouless energy. The experimental variations strikingly follow a universal law, close to the predictions of the proximity effect both in the long and short junction regime, as well as in the crossover region, thereby revealing the interplay of the different energy scales. Differences in the numerical coefficients reveal the crucial role played by the interfacial barrier between graphene and the superconducting electrodes, which reduces the supercurrent in both short and long junctions. Surprisingly the reduction of supercurrent is independent of the gate voltage and of the nature of the electrodes. A reduced induced gap and Thouless energy are extracted, revealing the role played by the dwell time in the barrier in the short junction, and an effective increased diffusion time in the long junction. We compare our results to the theoretical predictions of Usadel equations and numerical simulations which better reproduce experiments with imperfect NS interfaces.",1602.01489v1 2016-02-16,An Integrated Tantalum Sulfide - Boron Nitride - Graphene Oscillator: A Charge-Density-Wave Device Operating at Room Temperature,"The charge-density-wave (CDW) phase is a macroscopic quantum state consisting of a periodic modulation of the electronic charge density accompanied by a periodic distortion of the atomic lattice in quasi-1D or layered 2D metallic crystals. Several layered transition metal dichalcogenides, such as 1T-TaSe2, 1T-TaS2 and 1T-TiSe2, exhibit unusually high transition temperatures to different CDW symmetry-reducing phases. These transitions can be affected by environmental conditions, film thickness and applied electric bias. However, device applications of these intriguing systems at room temperature or their integration with other 2D materials have not been explored. Here we show that in 2D CDW 1T-TaS2, the abrupt change in the electrical conductivity and hysteresis at the transition point between nearly-commensurate and incommensurate charge-density-wave phases can be used for constructing an oscillator that operates at room temperature. The hexagonal boron nitride was capped on 1T-TaS2 thin film to provide protection from oxidation, and an integrated graphene transistor provides a voltage tunable, matched, low-resistance load enabling precise voltage control of the oscillator frequency. The integration of these three disparate two-dimensional materials, in a way that exploits the unique properties of each, yields a simple, miniaturized, voltage-controlled oscillator device. Theoretical considerations suggest that the upper limit of oscillation frequency to be in the THz regime.",1602.05147v1 2016-05-05,"Structural, optical and complex impedance spectroscopy study of multiferroic Bi2Fe4O9 ceramic","Multiferroic bismuth ferrite Bi_2Fe_4O_9 (BFO) ceramic was synthesized by conventional solid state reaction route. X-ray diffraction and Rietveld refinement show formation of single phase ceramic with orthorhombic crystal structure (space group Pbam). The morphological study depicted a well-defined grain of size $\simeq$2{\mu}m. The optical studies were carried out by using UV-Vis spectrophotometer which shows a band gap of 1.53 eV and a green emission spectrum at 537 is observed in the Photoluminescence study. The frequency dependent dielectric study at various temperature revealed that the dielectric constant decreases with increase in frequency. A noticeable peak shift towards higher frequency with increasing temperature is observed in the frequency dependent dielectric loss plot. The impedance spectroscopy shows a substantial shift in imaginary impedance (Z"") peaks toward the high frequency side described that the conduction in material favoring the long range motion of mobile charge carriers. The presence of non-Debye type multiple relaxations has been confirmed by complex modulus analysis. The frequency dependent ac conductivity at different temperatures indicates that the conduction process is thermally activated. The variation of dc conductivity exhibited a negative temperature coefficient of resistance behavior. The activation energy calculated from impedance, modulus and conductivity data confirmed that the oxygen vacancies play a vital role in the conduction mechanism.",1605.01574v1 2016-08-24,Engineering quantum spin Hall insulators by strained-layer heterostructures,"Quantum spin Hall insulators (QSHIs), also known as two-dimensional topological insulators, have emerged as an unconventional class of quantum states with insulating bulk and conducting edges originating from nontrivial inverted band structures, and have been proposed as a platform for exploring spintronics applications and exotic quasiparticles related to the spin-helical edge modes. Despite theoretical proposals for various materials, however, experimental demonstrations of QSHIs have so far been limited to two systems--HgTe/CdTe and InAs/GaSb--both of which are lattice-matched semiconductor heterostructures. Here we report transport measurements in yet another realization of a band-inverted heterostructure as a QSHI candidate--InAs/In$_{x}$Ga$_{1-x}$Sb with lattice mismatch. We show that the compressive strain in the In$_{x}$Ga$_{1-x}$Sb layer enhances the band overlap and energy gap. Consequently, high bulk resistivity, two orders of magnitude higher than for InAs/GaSb, is obtained deep in the band-inverted regime. The strain also enhances bulk Rashba spin-orbit splitting, leading to an unusual situation where the Fermi level crosses only one spin branch for electronlike and holelike bands over a wide density range. These properties make this system a promising platform for robust QSHIs with unique spin properties and demonstrate strain to be an important ingredient for tuning spin-orbit interaction.",1608.06751v2 2016-11-29,Magnetoelectric effect in antiferromagnetic multiferroic Pb(Fe1/2Nb1/2)O3 and its solid solutions with PbTiO3,"Antiferromagnets (AFMs) are presently considered as promising materials for applications in spintronics and random access memories due to the robustness of information stored in AFM state against perturbing magnetic fields (P. Wadley et al., Science 351, 587 (2016)). In this respect, AFM multiferroics maybe attractive alternatives for conventional AFMs as the coupling of magnetism with ferroelectricity (magnetoelectric effect) offers an elegant possibility of electric field control and switching of AFM domains. Here we report the results of comprehensive experimental and theoretical investigations of the quadratic magnetoelectric (ME) effect in single crystals and high-resistive ceramics of Pb(Fe1/2Nb1/2)O3 (PFN) and (1- x)Pb(Fe1/2Nb1/2)O3xPbTiO3 (PFNxPT). We are interested primarily in the temperature range of multiferroic phase, T < 150 K, where the ME coupling coefficient is extremely large (as compared to well-known multiferroic BiFeO3) and shows sign reversal at paramagnetic-to-antiferromagnetic phase transition. Moreover, we observe strong ME response nonlinearity in the AFM phase in the magnetic fields of only few kOe. To describe the temperature and magnetic field dependencies of the above unusual features of ME effect in PFN and PFN-xPT, we use simple phenomenological Landau approach which explains experimental data surprisingly well. Our ME measurements demonstrate that the electric field of only 20-25 kV/cm is able to switch the AFM domains and align them with ferroelectric ones even in PFN ceramic samples.",1611.09899v1 2017-11-21,Nanofeatures Induced by Severe Shot Peening (SSP) on Magnesium Alloy AZ31,"Considering the sensitivity of both fatigue strength and corrosion rate to the surface characteristics, apposite surface treatments could address the related challenges for biodegradable magnesium-based materials. Herein, we treated the surface of a biocompatible magnesium alloy by a low cost and versatile severe plastic deformation technique, severe shot peening, to evaluate the potential of surface grain refinement to enhance functionality in biological environment. The evolution of surface grain structure and surface morphology were investigated using optical as well as scanning and transmission electron microscopy. Surface roughness, wettability and chemical composition, as well as in depth-microhardness and residual stress distribution, and corrosion resistance were investigated. Successive light surface grinding was used after severe shot peening to eliminate the effect of surface roughness and separately investigate the influence of grain refinement alone. Cytocompatibility tests with osteoblasts (or bone forming cells) were performed using sample extracts. Results revealed for the first time that severe shot peening can significantly enhance mechanical properties without causing adverse effects to the growth of surrounding osteoblasts. The corrosion behavior, on the other hand, was not improved by severe shot peening; nevertheless, slight grinding of the rough surface layer with a high density of crystallographic lattice defects, without removing the entire nanocrystallized layer, provided a good potential for improving corrosion characteristics after severe shot peening and thus, this method should be studied for a wide range of orthopedic applications in which biodegradable magnesium is used.",1712.02834v1 2017-12-13,Quantum effects on dislocation motion from Ring-Polymer Molecular Dynamics,"Quantum motion of atoms known as zero-point vibrations is recognized to be important at low temperatures in condensed matter systems comprised of light atoms or ions, affecting such properties and behaviors as proton-transfer reactions, vibrational spectra of water and ice, and mechanical properties of low temperature helium. Recently, quantum motion of atoms was proposed to explain a long-standing discrepancy between theoretically computed and experimentally measured low-temperature resistance (Peierls stress) to dislocation motion in iron and possibly other metals with high atomic masses. Here we report the first direct simulations of quantum motion of screw dislocations in iron within the exact formalism of Ring-Polymer Molecular Dynamics (RPMD) that rigorously accounts for quantum effects on the statistics of condensed-phase systems. Our quantum RPMD simulations predict only a modest ($\approx\!13\%$) reduction in the Peierls stress in iron compared to its fully classical prediction. Our simulations confirm that reduction in the Peierls stress solely due to the zero-point energy is close to $50\%$ predicted earlier, but its effect is substantially offset by an increase in the effective atom size with decreasing temperature, an effect known as quantum dispersion. Thus, quantum motion of atoms does not resolve the notorious discrepancy between theoretical and experimental values of the Peierls stress in iron.",1712.04629v2 2018-02-06,Quasiparticle dynamics in granular aluminum close to the superconductor to insulator transition,"Superconducting high kinetic inductance elements constitute a valuable resource for quantum circuit design and millimeter-wave detection. Granular aluminum (GrAl) in the superconducting regime is a particularly interesting material since it has already shown a kinetic inductance in the range of nH$/\Box$ and its deposition is compatible with conventional Al/AlOx/Al Josephson junction fabrication. We characterize microwave resonators fabricated from GrAl with a room temperature resistivity of $4 \times 10^3\,\mu\Omega\cdot$cm, which is a factor of 3 below the superconductor to insulator transition, showing a kinetic inductance fraction close to unity. The measured internal quality factors are on the order of $Q_{\mathrm{i}} = 10^5$ in the single photon regime, and we demonstrate that non-equilibrium quasiparticles (QP) constitute the dominant loss mechanism. We extract QP relaxation times in the range of 1 s and we observe QP bursts every $\sim 20$ s. The current level of coherence of GrAl resonators makes them attractive for integration in quantum devices, while it also evidences the need to reduce the density of non-equilibrium QPs.",1802.01858v2 2018-01-06,Apically Dominant Mechanism for Improving Catalytic Activities of N-Doped Carbon Nanotube Arrays in Rechargeable Zinc-Air Battery,"The oxygen reduction (ORR) and oxygen evolution reactions (OER) in Zn-air batteries (ZABs) require highly efficient, cost-effective and stable electrocatalysts as replacements to traditionally high cost, inconsistently stable and low poison resistant Platinum group metals (PGM) catalysts. Although, nitrogen-doped carbon nanotube (NCNT) arrays have been developed over recent decades through various advanced technologies are now capable of catalyzing ORR efficiently, their underdeveloped bifunctional property, hydrophobic surface, and detrimental preparation strategy are found to limit practical large-scale commercialization for effective rechargeable ZABs. Here, we have demonstrated fabrication of a three-dimensional (3D) nickel foam supported NCNT arrays with CoNi nanoparticles (NPs) encapsulated within the apical domain (denoted as CoNi@NCNT/NF) that exhibits excellent bifunctional catalytic performance toward both ORR (onset potential of 0.97 V vs. RHE) and OER (overpotential of 1.54 V vs. RHE at 10 mA cm$^{-2}$). We further examined the practicability of this CoNi@NCNT/NF material being used as an air electrode for rechargeable ZAB coin cell and pouch cell systems. The ZAB coin cell showed a peak power density of 108 mW cm$^{-2}$ with an energy density of 845 Wh kg$_{Zn}^{-1}$ and robust rechargeability over 28h under ambient conditions, which exceeds the performance of PGM catalysts and leading non-PGM electrocatalysts. In addition, density functional theory (DFT) calculations revealed that the ORR and OER catalytic performance of the CoNi@NCNT/NF electrode are mainly derived from the d-orbitals from the CoNi NPs encapsulated within the apical dominant end of the NCNTs.",1802.02063v1 2018-03-06,Magic-angle graphene superlattices: a new platform for unconventional superconductivity,"The understanding of strongly-correlated materials, and in particular unconventional superconductors, has puzzled physicists for decades. Such difficulties have stimulated new research paradigms, such as ultra-cold atom lattices for simulating quantum materials. Here we report on the realization of intrinsic unconventional superconductivity in a 2D superlattice created by stacking two graphene sheets with a small twist angle. For angles near $1.1^\circ$, the first `magic' angle, twisted bilayer graphene (TBG) exhibits ultra-flat bands near charge neutrality, which lead to correlated insulating states at half-filling. Upon electrostatic doping away from these correlated insulating states, we observe tunable zero-resistance states with a critical temperature $T_c$ up to 1.7 K. The temperature-density phase diagram shows similarities with that of the cuprates, including superconducting domes. Moreover, quantum oscillations indicate small Fermi surfaces near the correlated insulating phase, in analogy with under-doped cuprates. The relative high $T_c$, given such small Fermi surface (corresponding to a record-low 2D carrier density of $10^{11} \textrm{cm}^{-2}$ , renders TBG among the strongest coupling superconductors, in a regime close to the BCS-BEC crossover. These novel results establish TBG as the first purely carbon-based 2D superconductor and as a highly tunable platform to investigate strongly-correlated phenomena, which could lead to insights into the physics of high-$T_c$ superconductors and quantum spin liquids.",1803.02342v2 2018-03-31,The Role of Crystal Orientation in the Dissolution of UO$_2$ Thin Films,"Epitaxial thin films have been utilised to investigate the radiolytic dissolution of uranium dioxide interfaces. Thin films of UO$_2$ deposited on single crystal yttria stabilised zirconia substrates have been exposed to water in the presence of a high flux, monochromatic, synchrotron x-ray source. In particular, this technique was applied to induce dissolution of three UO$_2$ thin films, grown along the principle UO$_2$ crystallographic orientations: (001), (110) and (111). Dissolution of each film was induced for 9 accumulative corrosion periods, totalling 270s, after which XRR spectra were recorded to observe the change in morphology of the films as a function of exposure time. While the (001) and (110) oriented films were found to corrode almost linearly and at comparable rates, the (111) film was found to be significantly more corrosion resistant, with no loss of UO$_2$ material being observed after the initial 90s corrosion period. These results distinctly show the effect of crystallographic orientation on the rate of x-ray induced UO$_2$ dissolution. This result may have important consequences for theoretical dissolution models, as it is evident that orientation dependence must be taken into consideration to obtain accurate predictions of the dissolution behaviour of UO$_2$.",1804.00201v1 2018-05-24,Impact of thermal fluctuations on transport in antiferromagnetic semimetals,"Recent demonstrations on manipulating antiferromagnetic (AF) order have triggered a growing interest in antiferromagnetic metal (AFM), and potential high-density spintronic applications demand further improvements in the anisotropic magnetoresistance (AMR). The antiferromagnetic semimetals (AFS) are newly discovered materials that possess massless Dirac fermions that are protected by the crystalline symmetries. In this material, a reorientation of the AF order may break the underlying symmetries and induce a finite energy gap. As such, the possible phase transition from the semimetallic to insulating phase gives us a choice for a wide range of resistance ensuring a large AMR. To further understand the robustness of the phase transition, we study thermal fluctuations of the AF order in AFS at a finite temperature. For macroscopic samples, we find that the thermal fluctuations effectively decrease the magnitude of the AF order by renormalizing the effective Hamiltonian. Our finding suggests that the insulating phase exhibits a gap narrowing at elevated temperatures, which leads to a substantial decrease in AMR. We also examine spatially correlated thermal fluctuations for microscopic samples by solving the microscopic Landau-Lifshitz-Gilbert equation finding a qualitative difference of the gap narrowing in the insulating phase. For both cases, the semimetallic phase shows a minimal change in its transmission spectrum illustrating the robustness of the symmetry protected states in AFS. Our finding may serve as a guideline for estimating and maximizing AMR of the AFS samples at elevated temperatures.",1805.09826v1 2018-09-03,Imparting icephobicity with substrate flexibility,"Ice accumulation hinders the performance of, and poses safety threats for infrastructure both on the ground and in the air. Previously, rationally designed superhydrophobic surfaces have demonstrated some potential as a passive means to mitigate ice accretion; however, further studies on material solutions that reduce impalement and contact time for impacting supercooled droplets and can also repel droplets that freeze during surface contact are urgently needed. Here we demonstrate the collaborative effect of substrate flexibility and surface nanotexture on enhancing both icephobicity and the repellency of viscous droplets. We first investigate the influence of increased viscosity on impalement resistance and droplet-substrate contact time after impact. Then we examine the effect of droplet partial solidification on recoil and simulate more challenging icing conditions by impacting supercooled water droplets onto flexible and rigid surfaces containing ice nucleation promoters. We demonstrate a passive mechanism for shedding partially solidified droplets under conditions where partial solidification occurs much faster than the natural droplet oscillation which does not rely on converting droplet surface energy into kinetic energy. Using an energy-based model, we identify a previously unexplored mechanism whereby the substrate oscillation and velocity govern the rebound process, with low-areal density and moderately stiff substrates acting to efficiently absorb the incoming droplet kinetic energy and rectify it back, allowing droplets to overcome adhesion and gravitational forces, and recoil. This mechanism applies for a range of droplet viscosities, spanning from low to high viscosity fluids and even ice slurries, which do not rebound from rigid superhydrophobic substrates.",1809.00490v1 2018-11-12,Antiferromagnet-based spintronic functionality by controlling isospin domains in a layered perovskite iridate,"The novel electronic state of the canted antiferromagnetic (AFM) insulator, strontium iridate (Sr2IrO4) has been well described by the spin-orbit-entangled isospin Jeff = 1/2, but the role of isospin in transport phenomena remains poorly understood. In this study, antiferromagnet-based spintronic functionality is demonstrated by combining unique characteristics of the isospin state in Sr2IrO4. Based on magnetic and transport measurements, large and highly anisotropic magnetoresistance (AMR) is obtained by manipulating the antiferromagnetic isospin domains. First-principles calculations suggest that electrons whose isospin directions are strongly coupled to in-plane net magnetic moment encounter the isospin mismatch when moving across antiferromagnetic domain boundaries, which generates a high resistance state. By rotating a magnetic field that aligns in-plane net moments and removes domain boundaries, the macroscopically-ordered isospins govern dynamic transport through the system, which leads to the extremely angle-sensitive AMR. As with this work that establishes a link between isospins and magnetotransport in strongly spin-orbit-coupled AFM Sr2IrO4, the peculiar AMR effect provides a beneficial foundation for fundamental and applied research on AFM spintronics.",1811.04562v1 2018-11-30,Spin Gapless Semiconducting Nature in Co-rich Co1+xFe1-xCrGa: Insight and Advancements,"In this report, we present structural, electronic, magnetic and transport properties of Co-rich spin gapless semiconductor CoFeCrGa using both theoretical and experimental techniques. The key advantage of Co-rich samples $\mathrm{Co_{1+x}Fe_{1-x}CrGa}$ is the high Curie temperature (T$\mathrm{_C}$) and magnetization, without compromising the SGS nature (up to x = 0.4), and hence our choice. The quaternary Heusler alloys $\mathrm{Co_{1+x}Fe_{1-x}CrGa}$ (x = 0.1 to 0.5) are found to crystallize in LiMgPdSn-type structure having space group $F\bar{4}3m$ (\# 216). The measured Curie temperature increases from 690 K (x = 0) to 870 K (x = 0.5). Observed magnetization values follow the Slater-Pauling rule. Measured electrical resistivity, in the temperature range of 5-350 K, suggests that the alloys retain the SGS behavior up to x = 0.4, beyond which it reflects metallic character. Unlike conventional semiconductors, the conductivity value ($\mathrm{\sigma_{xx}}$) at 300 K lies in the range of 2289 S $\mathrm{cm^{-1}}$ to 3294 S $\mathrm{cm^{-1}}$, which is close to that of other reported SGS materials. The anomalous Hall effect is comparatively low. The intrinsic contribution to the anomalous Hall conductivity increase with x, which can be correlated with the enhancement in chemical order. The anomalous Hall coefficient is found to increase from 38 S/cm for x = 0.1 to 43 S/cm for 0.3. Seebeck coefficients turn out to be vanishingly small below 300 K, another signature for being SGS. All the alloys (for different x) are found to be both chemically and thermally stable. Simulated magnetization agrees fairly with the experiment. As such Co-rich CoFeCrGa is a promising candidate for room temperature spintronic applications, with enhanced T$\mathrm{_C}$, magnetic properties and SGS nature.",1811.12684v1 2019-09-24,Spin-transfer dynamics in MgO-based magnetic tunnel junctions with an out-of-plane magnetized free layer and an in-plane polarizer,"Here, we present an analytical and numerical model describing the magnetization dynamics in MgO-based spin-torque nano-oscillators with an in-plane magnetized polarizer and an out-of-plane free layer. We introduce the spin-transfer torque asymmetry by considering the cosine angular dependence of the resistance between the two magnetic layers in the stack. For the analytical solution, dynamics are determined by assuming a circular precession trajectory around the direction perpendicular to the plane, as set by the effective field, and calculating the energy integral over a single precession period. In a more realistic approach, we include the bias dependence of the tunnel magnetoresistance, which is assumed empirically to be a piecewise linear function of the applied voltage. The dynamical states are found by solving the stability condition for the Jacobian matrix for out-of-plane static states. We find that the bias dependence of the tunnel magnetoresistance, which is an inseparable effect in every tunnel junction, exhibits drastic impact on the spin-torque nano-oscillator phase diagram, mainly by increasing the critical current for dynamics and quenching the oscillations at high currents. The results are in good agreement with our experimental data published elsewhere.",1909.10983v1 2020-03-16,Unconventional Hall response in the quantum limit of HfTe5,"Interacting electrons confined to their lowest Landau level in a high magnetic field can form a variety of correlated states, some of which manifest themselves in a Hall effect. Although such states have been predicted to occur in three dimensional semimetals, a corresponding Hall response has not yet been experimentally observed. Here, we report the observation of an unconventional Hall response in the quantum limit of the bulk semimetal HfTe5, adjacent to the three-dimensional quantum Hall effect of a single electron band at low magnetic fields. The additional plateau-like feature in the Hall conductivity of the lowest Landau level is accompanied by a Shubnikov-de Haas minimum in the longitudinal electrical resistivity and its magnitude relates as 3/5 to the height of the last plateau of the three-dimensional quantum Hall effect. Our findings are consistent with strong electron-electron interactions, stabilizing an unconventional variant of the Hall effect in a three-dimensional material in the quantum limit.",2003.07213v3 2017-03-07,Fast multicolor photodetectors based on graphene-contacted p-GaSe/n-InSe van der Waals heterostructures,"The integration of different two-dimensional materials within a multilayer van der Waals (vdW) heterostructure offers a promising technology for realizing high performance opto-electronic devices such as photodetectors and light sources1-3. Transition metal dichalcogenides, e.g. MoS2 and WSe2, have been employed as the optically-active layer in recently developed heterojunctions. However, MoS2 and WSe2 become direct band gap semiconductors only in mono- or bilayer form4,5. In contrast, the metal monochalcogenides InSe and GaSe retain a direct bandgap over a wide range of layer thicknesses from bulk crystals down to exfoliated flakes only a few atomic monolayers thick6,7. Here we report on vdW heterojunction diodes based on InSe and GaSe: the type II band alignment between the two materials and their distinctive spectral response, combined with the low electrical resistance of transparent graphene electrodes, enable effective separation and extraction of photoexcited carriers from the heterostructure even when no external voltage is applied. Our devices are fast (< 10 {\mu}s), self-driven photodetectors with multicolor photoresponse ranging from the ultraviolet to the near-infrared and have the potential to accelerate the exploitation of two-dimensional vdW crystals by creating new routes to miniaturized optoelectronics beyond present technologies.",1703.02534v1 2017-03-28,Co-appearance of superconductivity and ferromagnetism in a Ca$_2$RuO$_4$ nanofilm crystal,"By tuning the physical and chemical pressures of layered perovskite materials we can realize the quantum states of both superconductors and insulators. By reducing the thickness of a layered crystal to a nanometer level, a nanofilm crystal can provide novel quantum states that have not previously been found in bulk crystals. Here we report the realization of high-temperature superconductivity in Ca$_2$RuO$_4$ nanofilm single crystals. Ca$_2$RuO$_4$ thin film with the highest transition temperature $T_c$ (midpoint) of 64~K exhibits zero resistance in electric transport measurements. The superconducting critical current exhibited a logarithmic dependence on temperature and was enhanced by an external magnetic field. Magnetic measurements revealed a ferromagnetic transition at 180~K and diamagnetic magnetization due to superconductivity. Our results suggest the co-appearance of superconductivity and ferromagnetism in Ca$_2$RuO$_4$ nanofilm crystals. We also found that the induced bias current and the tuned film thickness caused a superconductor-insulator transition. The fabrication of micro-nanocrystals made of layered material enables us to discuss rich superconducting phenomena in ruthenates.",1703.09459v2 2018-10-16,The superconductor-superinsulator transition: S-duality and QCD on the desktop,"We show that the nature of quantum phases around the superconductor-insulator transition (SIT) is controlled by charge-vortex topological interactions and does not depend on the details of material parameters and disorder. We find three distinct phases, superconductor, superinsulator and bosonic topological insulator. The superinsulator is a state of matter with infinite resistance in a finite temperature range, which is the S-dual of the superconductor and in which charge transport is prevented by electric strings binding charges of opposite sign. The electric strings ensuring linear confinement of charges are generated by instantons and are dual to superconducting Abrikosov vortices. Material parameters and disorder enter the London penetration depth of the superconductor, the string tension of the superinsulator and the quantum fluctuation parameter driving the transition between them. They are entirely encoded in four phenomenological parameters of a topological gauge theory of the SIT. Finally, we point out that, in the context of strong coupling gauge theories, the many-body localization phenomenon that is often referred to as an underlying mechanism for superinsulation is a mere transcription of the well-known phenomenon of confinement into solid state physics language and is entirely driven by endogenous disorder embodied by instantons with no need of exogenous disorder.",1810.06862v1 2020-04-14,Intrinsically Activated SrTiO3: Photocatalytic H2 Evolution from Neutral Aqueous Methanol Solution in the Absence of Any Noble Metal Cocatalyst,"Noble metal cocatalysts are conventionally a crucial factor in oxide-semiconductor-based photocatalytic hydrogen generation. In the present work, we show that optimized high-temperature hydrogenation of commercially available strontium titanate (SrTiO3) powder can be used to engineer an intrinsic cocatalytic shell around nanoparticles that can create a photocatalyst that is highly effective without the use of any additional cocatalyst for hydrogen generation from neutral aqueous methanol solutions. This intrinsic activation effect can also be observed for SrTiO3[100] single crystal as well as Nb-doped SrTiO3 (100) single crystal. For all types of SrTiO3 samples (nanopowders and either of the single crystals), hydrogenation under optimum conditions leads to a surface-hydroxylated layer together with lattice defects visible by transmission electron microscopy, electron paramagnetic resonance (EPR), and photoluminescence (PL). Active samples provide states in a defective matrix -- this is in contrast to the inactive defects formed in other reductive atmospheres. In aqueous media, active SrTiO3 samples show a significant negative shift of the flatband potential (in photoelectrochemical as well as in capacitance data) and a lower charge-transfer resistance for photoexcited electrons. We therefore ascribe the remarkable cocatalyst-free activation of the material to a synergy between thermodynamics (altered interface energetics induced by hydroxylation) and kinetics (charge transfer mediation by suitable Ti3+ states).",2004.06573v1 2022-02-10,Dynamics of Multi-Domains in Ferroelectric Tunnel Junction,"The Discovery of giant tunnel electroresistance (TER) in Ferroelectric Tunnel Junction (FTJ) paves a futuristic possibility of utilizing the FTJ as a bistable resistive device with an enormously high ON/OFF ratio. In the last 20 years, numerous studies have reported that the formation of multidomain in ferroelectric material is an inevitable process to minimize the total system energy. Recent studies based on phase-field simulations have demonstrated that domain nucleation/motion substantially alters the electrostatics of a ferroelectric material. However, the impact of domain dynamics on quantum transport in FTJ remains elusive. This paper presents a comprehensive study of multidomain dynamics in a ferroelectric tunnel junction. Analysis of this article is twofold; firstly, we study the impact of domain dynamics on electrostatics in an FTJ. Subsequently, the obtained electrostatics is used to study the variations in tunneling current, and TER originated from multidomain dynamics. We show that ON/OFF current density and TER vary locally in the ferroelectric region. Furthermore, the device's electrostatics and quantum transport exhibit an oscillatory nature due to periodic domain texture. ON/OFF current density shows a sine/cosine distribution in ferroelectric, and approximately one-decade local variation in current density is observed. These local fluctuations in current density cause oscillations in the device's ON/OFF ratio. Optimization techniques to achieve a uniform and maximum TER are also discussed. A 2D analytical and explicit model is derived by solving coupled 2D Poisson's equation and Landau-Ginzburg equation. The model incorporates the switching and nucleation of domains by minimizing net ferroelectric energy (depolarization+free+gradient energy density). Furthermore, the impact of the bottom insulator layer on ferroelectric's gradient energy is also studied.",2202.04926v1 2022-02-15,A Ta-TaS2 monolithic catalyst with robust and metallic interface for superior hydrogen evolution,"The use of highly active and robust catalysts is crucial for producing green hydrogen by water electrolysis as we strive to achieve global carbon neutrality. Noble metals like platinum are currently used in industry for the hydrogen evolution reaction (HER), but suffer from scarcity, high price and unsatisfied performance and stability at large current density, restricting their large scale implementations. Here we report the synthesis of a new type of monolithic catalyst (MC) consisting of a metal disulfide (e.g., TaS2) catalyst vertically bonded to a conductive substrate of the same metal by strong covalent bonds. These features give the MC a mechanically robust and electrically near zero resistance interface, leading to an outstanding HER performance including rapid charge transfer and excellent durability, together with a low overpotential of 398 mV to achieve a current density of 2,000 mA cm-2 as required by industry. The Ta TaS2 MC has a negligible performance decay after 200 h operation at large current densities. In light of its unique interface and the various choice of metal elements giving the same structure, such monolithic materials may have broad uses besides catalysis.",2202.07339v1 2017-04-19,Potential Fluctuations at Low Temperatures in Mesoscopic-Scale SmTiO$_{3}$/SrTiO$_{3}$/SmTiO$_{3}$ Quantum Well Structures,"Heterointerfaces of SrTiO$_{3}$ with other transition metal oxides make up an intriguing family of systems with a bounty of coexisting and competing physical orders. Some examples, such as LaAlO$_{3}$/SrTiO$_{3}$, support a high carrier density electron gas at the interface whose electronic properties are determined by a combination of lattice distortions, spin-orbit coupling, defects, and various regimes of magnetic and charge ordering. Here, we study electronic transport in mesoscale devices made with heterostructures of SrTiO$_{3}$ sandwiched between layers of SmTiO$_{3}$, in which the transport properties can be tuned from a regime of Fermi-liquid like resistivity ($\rho \sim T^{2}$) to a non-Fermi liquid ($\rho \sim T^{5/3}$) by controlling the SrTiO$_{3}$ thickness. In mesoscale devices at low temperatures, we find unexpected voltage fluctuations that grow in magnitude as $T$ is decreased below 20 K, are suppressed with increasing contact electrode size, and are independent of the drive current and contact spacing distance. Magnetoresistance fluctuations are also observed, which are reminiscent of universal conductance fluctuations but not entirely consistent with their conventional properties. Candidate explanations are considered, and a mechanism is suggested based on mesoscopic temporal fluctuations of the Seebeck coefficient. An improved understanding of charge transport in these model systems, especially their quantum coherent properties, may lead to insights into the nature of transport in strongly correlated materials that deviate from Fermi liquid theory.",1704.05744v1 2017-08-06,Electrical transport and optical band gap of NiFe$_\textrm{2}$O$_\textrm{x}$ thin films,"We fabricated NiFe$_\textrm{2}$O$_\textrm{x}$ thin films on MgAl$_2$O$_4$(001) substrates by reactive dc magnetron co-sputtering varying the oxygen partial pressure during deposition. The fabrication of a variable material with oxygen deficiency leads to controllable electrical and optical properties which would be beneficial for the investigations of the transport phenomena and would, therefore, promote the use of such materials in spintronic and spin caloritronic applications. We used several characterization techniques in order to investigate the film properties, focusing on their structural, magnetic, electrical, and optical properties. From the electrical resistivity measurements we obtained the conduction mechanisms that govern the systems in high and low temperature regimes, extracting low thermal activation energies which unveil extrinsic transport mechanisms. The thermal activation energy decreases in the less oxidized samples revealing the pronounced contribution of a large amount of electronic states localized in the band gap to the electrical conductivity. Hall effect measurements showed the mixed-type semiconducting character of our films. The optical band gaps were determined via ultraviolet-visible spectroscopy. They follow a similar trend as the thermal activation energy, with lower band gap values in the less oxidized samples.",1708.01937v1 2019-03-05,All-optical cryogenic thermometry based on NV centers in nanodiamonds,"The nitrogen-vacancy (NV) center in diamond has been recognized as a high-sensitivity nanometer-scale metrology platform. Thermometry has been a recent focus, with attention largely confined to room temperature applications. Thermometry has been a recent focus, with attention largely confined to room temperature applications. Temperature sensing at low temperatures, however, remains challenging as the sensitivity decreases for many commonly used techniques which rely on a temperature dependent frequency shift of the NV centers spin resonance and its control with microwaves. Here we use an alternative approach that does not require microwaves, ratiometric all-optical thermometry, and demonstrate that it may be utilized to liquid nitrogen temperatures without deterioration of the sensitivity. The use of an array of nanodiamonds embedded within a portably polydimethylsiloxane (PDMS) sheet provides a versatile temperature sensing platform that can probe a wide variety of systems without the configurational restrictions needed for applying microwaves. With this device, we observe a temperature gradient over tens of microns in a ferromagnetic-insulator substrate (YIG) under local heating by a resistive heater. This thermometry technique provides a cryogenically compatible, microwave-free, minimally invasive approach capable of probing local temperatures with few restrictions on the substrate materials.",1903.01605v1 2021-01-03,3D Fluorescent Mapping of Invisible Molecular Damage after Cavi-tation in Hydrogen Exposed Elastomers,"Elastomers saturated with gas at high pressure suffer from cavity nucleation, inflation, and deflation upon rapid or explosive de-compression. Although this process often results in undetectable changes in appearance, it causes internal damage, hampers func-tionality (e.g., permeability), and shortens lifetime. Here, we tag a model poly(ethyl acrylate) elastomer with {\pi}-extended anthracene-maleimide adducts that fluoresce upon polymer chain scission, and map in 3D the internal damage present after a cycle of gas satu-ration and rapid decompression. Interestingly, we observe that each cavity observable during the decompression results in a dam-aged region, the shape of which reveals a fracture locus of randomly oriented penny-shape cracks (i.e., with a flower-like morpholo-gy) that contain crack arrest lines. Thus, cavity growth likely proceeds discontinuously (i.e., non-steadily) through the stable and unstable fracture of numerous 2D crack planes. This non-destructive methodology to visualize in 3D molecular damage in polymer networks is novel and serves to understand how fracture occurs under complex 3D loads, predict mechanical aging of pristine look-ing elastomers, and holds potential to optimize cavitation-resistant materials.",2101.00709v2 2021-01-28,Macroscopic yarns of FeCl$_{3}$-intercalated collapsed carbon nano-tubes with high doping and stability,"Macroscopic arrays of highly crystalline nanocarbons offer the possibility of modifying the electronic structure of their low dimensional constituents, for example through doping, and studying the resulting collective bulk behaviour. Insertion of electron donors or acceptors between graphitic layers is an attractive method to reversibly increase charge carrier concentra-tion without disruption of the sp$2$-conjugated system. This work demonstrates FeCl$_{3}$ intercalation into fibres made up of collapsed (flattened) carbon nanotubes. The bundles of collapsed CNTs, similar to crystallites of graphitic nanoribbons, host elongated layered FeCl$_{3}$ crystals of hundreds of $nm$ long, much longer than previous reports on graphitic materials and directly observable by transmission electron microscopy and X-ray diffraction. Intercalated CNT fibres remain stable after months of exposure to ambient conditions, partly due to the spontaneous formation of passivating monolayers of FeClO at the crystal edge, preventing both desorption of intercalant and further hydrolysis. Raman spectroscopy shows substantial electron transfer from the CNTs to FeCl$_{3}$, a well-known acceptor, as observed by G band upshifts as large as $25 cm^{-1}$. After resolving Raman features for the inner and outer layers of the collapsed CNTs, strain and dynamic effect contributions of charge transfer to the Raman upshift could be decoupled, giving a Fermi level downshift of $- 0.72 eV$ and a large average free carrier concentration of $5.3X10^{13}$ $cm^{-2}$ ($0.014$ electrons per carbon atom) in the intercalated system. Four-probe resistivity measurements show an increase in conductivity by a factor of six upon intercalation",2101.12077v1 2021-01-29,Doping isolated one-dimensional antiferro-magnetic semiconductor Vanadium tetrasulfide ($VS_4$) nanowires with carriers induces half-metallicity,"Quasi one-dimensional (1D) vanadium tetrasulfide ($VS_4$) nanowires (NWs) are synthetic semiconductors which combine with each other through Van der Waals interactions to form bulk phases. However, the properties of these individual nanowires remain unknown. Nevertheless, our calculations of their stability indicate that $VS_4$) NWs can be separated from their bulk structures. Accordingly, we theoretically investigated the geometrical, electronic, and magnetic properties of bulk phase and isolated $VS_4$ NWs. Our results indicate that both bulk phase and isolated $VS_4$ NWs are semiconductors with band gaps of 2.24 and 2.64 eV, respectively, and that they prefer the antiferromagnetic (AFM) ground state based on DFT calculations. These calculations also suggested that isolated $VS_4$ NWs show half-metallic antiferromagnetism upon electron and hole doping because carrier doping splits the spin degeneracy to induce local spin polarisation. As a result, spin polarisation currents in isolated $VS_4$ NWs can be manipulated with locally applied gate voltage. Therefore, these 1D AFM materials have a high potential for advancing both fundamental research and spintronic applications because they are more resistant to magnetic perturbation than their 1D ferromagnetic counterparts.",2101.12658v1 2016-09-29,Quantum imaging of current flow in graphene,"Since its first isolation in 2004, graphene has been found to host a plethora of unusual electronic transport phenomena, making it a fascinating system for fundamental studies in condensed-matter physics as well as offering tremendous opportunities for future electronic and sensing devices. However, to fully realise these goals a major challenge is the ability to non-invasively image charge currents in monolayer graphene structures and devices. Typically, electronic transport in graphene has been investigated via resistivity measurements, however, such measurements are generally blind to spatial information critical to observing and studying landmark transport phenomena such as electron guiding and focusing, topological currents and viscous electron backflow in real space, and in realistic imperfect devices. Here we bring quantum imaging to bear on the problem and demonstrate high-resolution imaging of current flow in graphene structures. Our method utilises an engineered array of near-surface, atomic-sized quantum sensors in diamond, to map the vector magnetic field and reconstruct the vector current density over graphene geometries of varying complexity, from mono-ribbons to junctions, with spatial resolution at the diffraction limit and a projected sensitivity to currents as small as 1 {\mu}A. The measured current maps reveal strong spatial variations corresponding to physical defects at the sub-{\mu}m scale. The demonstrated method opens up an important new avenue to investigate fundamental electronic and spin transport in graphene structures and devices, and more generally in emerging two-dimensional materials and thin film systems.",1609.09208v1 2019-01-08,Quadratic to linear magnetoresistance tuning in TmB4,"The change of a material's electrical resistance (R) in response to an external magnetic field (B) provides subtle information for the characterization of its electronic properties and has found applications in sensor and storage related technologies. In good metals, Boltzmann's theory predicts a quadratic growth in magnetoresistance (MR) at low B, and saturation at high fields. On the other hand, a number of nonmagnetic materials with weak electronic correlation and low carrier concentration for metallicity, such as inhomogeneous conductors, semimetals, narrow gap semiconductors and topological insulators, two-dimensional electron gas (2DEG) show positive, non-saturating linear magnetoresistance (LMR). However, observation of LMR in single crystals of a good metal is rare. Here we present low-temperature, angle dependent magnetotransport in single crystals of the antiferromagnetic metal, TmB4. We observe large, positive and anisotropic MR(B), which can be tuned from quadratic to linear by changing the direction of the applied field. In view of the fact that isotropic, single crystalline metals with large Fermi surface (FS) are not expected to exhibit LMR, we attribute our observations to the anisotropic FS topology of TmB4. Furthermore, the linear MR is found to be temperature-independent, suggestive of quantum mechanical origin.",1901.02165v1 2019-01-30,Cathodoluminescence of CdZnSSe crystals synthesized in 19th century bead glass,"The article presents an experimental investigation of band-edge cathodoluminescence of CdZnSSe crystals that nucleated and grew in silicate glass melt during its production. We have studied Zn-rich red glass made for manufacture of seed beads in the 19th century and found it to contain CdZnSSe crystals. Due to colloidal staining using the CdZnSSe crystallites embedded in glass, glass makers were enabled to produce lustrous red glass that, as we presently know, manifests bright luminescence. The CdZnSSe crystallites exhibit intense band-edge cathodoluminescence both at room temperature and at liquid nitrogen temperature. We have found the band-edge cathodoluminescence of these crystals to peak in the range from 2.00 to 2.03 eV at 300 K and from 2.02 to 2.06 eV at 80 K. We have also estimated the value of the band gap derivative d$E_g$/d$T$ in the interval from 80 to 300 K and found it to lie in the range from $-2.5 \times 10^{-4}$ to 0 eV/K. CdZnSSe crystals in glass demonstrate high temperature and temporal stability. The glass-crystal composite on their basis is resistant to the electron-beam irradiation and long-term weathering. Possible applications of this composite in modern technologies, and processes and components that might be used for making glass stained with CdZnSSe in the past are also discussed.",1901.10764v3 2019-10-21,Revisiting Effects of Nitrogen Incorporation and Graphitization on Conductivity of Ultra-nano-crystalline Diamond Films,"Detailed structural and electrical properties of ultra-nano-crystalline diamond (UNCD) films grown in H$_\text{2}$/CH$_\text{4}$/N$_\text{2}$ plasma were systematically studied as a function of deposition temperature ($T_d$) and nitrogen content ($\%$ N$_2$) to thoroughly evaluate their effects on conductivity. $T_d$ was scanned from 1000 to 1300 K for N$_2$ fixed at 0, 5, 10 and 20 $\%$. It was found that even the films grown in the synthetic gas mixture with no nitrogen could be made as conductive as 1$-$10$^{-2}$ $\Omega$ cm with overall resistivity of all the films tuned over 4 orders of magnitude through varying growth parameters. On a set of 27 samples, Raman spectroscopy and scanning electron microscopy show a progressive and highly reproducible film material phase transformation, from ultra-nano-crystalline diamond to nano-crystalline graphite as deposition temperature increases. The rate of this transformation is heavily dependent on N$_2$ content. Addition of nitrogen greatly increases the amount of $sp^2$ bonded carbon in the films thus enhancing the physical connectivity in the GB network that have high electronic density of states. However, addition of nitrogen greatly slows down crystallization of $sp^2$ phase in the GBs. Therefore, proper balance between GB connectivity and crystallinity is the key in conductivity engineering of (N)UNCD.",1910.09595v1 2020-05-28,Powering Electronic Devices from Salt Gradients in AA Battery-Sized Stacks of Hydrogel-Infused Paper,"Strongly electric fish use gradients of ions within their bodies to generate stunning external electrical discharges; the most powerful of these organisms, the Atlantic torpedo ray, can produce pulses of over 1 kW from its electric organs. Despite extensive study of this phenomenon in nature, the development of artificial power generation schemes based on ion gradients for portable, wearable, or implantable human use has remained out of reach. Previously, inspired by the electric eel, we developed an artificial electric organ that generated electricity from ion gradients within stacked hydrogels and, like the eel, was optimized to deliver large voltages that exceeded 100 V. Due to its high internal resistance, the current of this power source was, however, too low to power standard electronics. Here we introduce an artificial electric organ that takes inspiration from the unique morphologies of torpedo rays for maximal current output. This power source uses a hybrid material of hydrogel-infused paper to create, organize, and reconfigure stacks of thin, arbitrarily large gel films both in series and in parallel. The resulting increase in electrical power by almost two orders of magnitude compared to the original eel-inspired design makes it possible to power electronic devices and establishes that biology's mechanism of generating significant electrical power can now be realized from benign and soft materials in a portable size.",2005.13775v1 2020-06-27,Controlling local resistance via electric-field induced dislocations,"Dislocations are one-dimensional (1D) topological line defects where the lattice deviates from the perfect crystal structure. The presence of dislocations transcends condensed matter research and gives rise to a diverse range of emergent phenomena [1-6], ranging from geological effects [7] to light emission from diodes [8]. Despite their ubiquity, to date, the controlled formation of dislocations is usually achieved via strain fields, applied either during growth [9,10] or retrospectively via deformation, e.g., (nano [11-14])-indentation [15]. Here we show how partial dislocations can be induced using local electric fields, altering the structure and electronic response of the material where the field is applied. By combining high-resolution imaging techniques and density functional theory calculations, we directly image these dislocations in the ferroelectric hexagonal manganite Er(Ti,Mn)O3 and study their impact on the local electric transport behaviour. The use of an electric field to induce partial dislocations is a conceptually new approach to the burgeoning field of emergent defect-driven phenomena and enables local property control without the need of external macroscopic strain fields. This control is an important step towards integrating and functionalising dislocations in practical devices for future oxide electronics.",2006.15252v1 2020-07-13,Approaching the Practical Conductivity Limits of Aerosol Jet Printed Silver,"Previous efforts to directly write conductive metals have been narrowly focused on nanoparticle ink suspensions that require aggressive sintering (>200 {\deg}C) and result in low-density, small-grained agglomerates with electrical conductivities <25% of bulk metal. Here, we demonstrate aerosol jet printing of a reactive ink solution and characterize high-density (93%) printed silver traces having near-bulk conductivity and grain sizes greater than the electron mean free path, while only requiring a low-temperature (80 {\deg}C) treatment. We have developed a predictive electronic transport model which correlates the microstructure to the measured conductivity and identifies a strategy to approach the practical conductivity limit for printed metals. Our analysis of how grain boundaries and tortuosity contribute to electrical resistivity provides insight into the basic materials science that governs how an ink formulator or process developer might approach improving the conductivity. Transmission line measurements validate that electrical properties are preserved up to 20 GHz, which demonstrates the utility of this technique for printed RF components. This work reveals a new method of producing robust printed electronics that retain the advantages of rapid prototyping and three-dimensional fabrication while achieving the performance necessary for success within the aerospace and communications industries.",2007.06645v1 2020-07-14,A phase field model for elastic-gradient-plastic solids undergoing hydrogen embrittlement,"We present a gradient-based theoretical framework for predicting hydrogen assisted fracture in elastic-plastic solids. The novelty of the model lies in the combination of: (i) stress-assisted diffusion of solute species, (ii) strain gradient plasticity, and (iii) a hydrogen-sensitive phase field fracture formulation, inspired by first principles calculations. The theoretical model is numerically implemented using a mixed finite element formulation and several boundary value problems are addressed to gain physical insight and showcase model predictions. The results reveal the critical role of plastic strain gradients in rationalising decohesion-based arguments and capturing the transition to brittle fracture observed in hydrogen-rich environments. Large crack tip stresses are predicted, which in turn raise the hydrogen concentration and reduce the fracture energy. The computation of the steady state fracture toughness as a function of the cohesive strength shows that cleavage fracture can be predicted in otherwise ductile metals using sensible values for the material parameters and the hydrogen concentration. In addition, we compute crack growth resistance curves in a wide variety of scenarios and demonstrate that the model can appropriately capture the sensitivity to: the plastic length scales, the fracture length scale, the loading rate and the hydrogen concentration. Model predictions are also compared with fracture experiments on a modern ultra-high strength steel, AerMet100. A promising agreement is observed with experimental measurements of threshold stress intensity factor $K_{th}$ over a wide range of applied potentials.",2007.07093v1 2020-07-16,Magnetotransport properties of the topological nodal-line semimetal CaCdSn,"Topological nodal-line semimetals support protected band crossings which form nodal lines or nodal loops between the valence and conduction bands and exhibit novel transport phenomena. Here we address the topological state of the nodal-line semimetal candidate material, CaCdSn, and report magnetotransport properties of its single crystals grown by the self-flux method. Our first-principles calculations show that the electronic structure of CaCdSn harbors a single nodal loop around the $\Gamma$ point in the absence of spin-orbit coupling (SOC) effects. The nodal crossings in CaCdSn are found to lie above the Fermi level and yield a Fermi surface that consists of both electron and hole pockets. CaCdSn exhibits high mobility ($\mu \approx 3.44\times 10^4$ cm$^2$V$^{-1}$s$^{-1}$) and displays a field-induced metal-semiconductor like crossover with a plateau in resistivity at low temperature. We observe an extremely large and quasilinear non-saturating transverse as well as longitudinal magnetoresistance (MR) at low temperatures ($\approx 7.44\times 10^3 \%$ and $\approx 1.71\times 10^3\%$, respectively, at 4K). We also briefly discuss possible reasons behind such a large quasilinear magnetoresistance and its connection with the nontrivial band structure of CaCdSn.",2007.08156v1 2020-07-27,Thermodynamic and corrosion study of Sm$_{1-x}$Mg$_x$Ni$_y$ (y = 3.5 or 3.8) compounds forming reversible hydrides,"AB5 compounds (A = rare earth, B = transition metal) have been widely studied as anodes for Ni-MH applications. However, they have reached their technical limitations and the search for new promising materials with high capacity is foreseen. ABy compounds (2 < y < 5) are good candidates. They are made by stacking [AB5] and [A2B4] units along the c crystallographic axis. The latter unit allows a large increase in capacity, while the [AB5] unit provides good cycling stability. Consequently, the AB3.8 composition (i.e. A5B19 with three [AB5] for one [A2B4]) is expected to exhibit better cycling stability than the AB3.5 (i.e. A2B7 with two [AB5] for one [A2B4]). Furthermore, substitution of rare earth by light magnesium improves both the capacity and cycling stability. In this paper, we compare the hydrogenation and corrosion properties of two binary compounds SmNi$_{3.5}$ and SmNi$_{3.8}$ and two pseudo-binary ones (Sm,Mg)Ni$_{3.5}$ and (Sm,Mg)Ni$_{3.8}$. A better solid-gas cycling stability is highlighted for the binary SmNi$_{3.8}$. The pseudo-binary compounds also exhibit higher cycling stability than the binary ones. Furthermore, their resistance to corrosion was investigated.",2007.13456v1 2020-08-12,"Investigation of the lead-free double perovskites Cs2AgSbX6 (X= Cl, Br, I) for optoelectronic and thermoelectric applications","Perovskite compounds have the potential to harvest solar energy as well as exploit the thermoelectric potential of a number of available materials. Here, we present the electronic, structural, thermoelectric, and optical properties of Cs2AgSbX6 (X = Cl, Br, I) perovskite with the help of the density functional theory (DFT). The WC-GGA approximation was used to calculate the structural parameters. All these compounds crystalize in a cubic unit cell with lattice constant increasing from 10.65 {\AA} (Cl) to 11.14 {\AA} (Br) to 11.86 {\AA} (I). The mBJ-functional shows a semiconducting nature for these compounds with an indirect band gap lying at the L-X symmetry points. The optical conductivity and absorption coefficient show their peaks in the ultraviolet region, moving towards a lower energy range by inserting large size anion. The band gap of these compounds (2.08, 1.37, 0.64 eV) indicates their potential in single and multijunction solar cells. The value of refractive index at zero energy was evaluated to be 3.1, 2.2, and 1.97 for Cs2AgSbCl6, Cs2AgSbBr6 and Cs2AgSbI6. Effective mass of electrons is smaller than those of holes resulting in higher carrier mobility for electrons. The Seebeck coefficient, power factor, and the figure of merit were computed using the BoltzTrap code. The negative temperature coefficient of resistivity also supports the semiconductor nature of these compounds. The high electrical, small thermal conductivity, positive Seebeck coefficient, and the optimum figure of merit make these compounds suitable for thermoelectric applications.",2008.06384v3 2020-08-27,Direct Imaging and Electronic Structure Modulation of Moiré Superlattices at the 2D/3D Interface,"The atomic structure at the interface between two-dimensional (2D) and three-dimensional (3D) materials influences properties such as contact resistance, photo-response, and high-frequency electrical performance. Moir\'e engineering is yet to be utilized for tailoring this 2D/3D interface, despite its success in enabling correlated physics at 2D/2D interfaces. Using epitaxially aligned MoS2/Au{111} as a model system, we demonstrate the use of advanced scanning transmission electron microscopy (STEM) combined with a geometric convolution technique in imaging the crystallographic 32 A moir\'e pattern at the 2D/3D interface. This moir\'e period is often hidden in conventional electron microscopy, where the Au structure is seen in projection. We show, via ab initio electronic structure calculations, that charge density is modulated according to the moir\'e period, illustrating the potential for (opto-)electronic moir\'e engineering at the 2D/3D interface. Our work presents a general pathway to directly image periodic modulation at interfaces using this combination of emerging microscopy techniques.",2008.12215v2 2020-10-08,"Microstructure, mechanical properties, corrosion resistance and cytocompatibility of WE43 Mg alloy scaffolds fabricated by laser powder bed fusion for biomedical applications","Open-porous scaffolds of WE43 Mg alloy with a body-center cubic cell pattern were manufactured by laser powder bed fusion with different strut diameters. The geometry of the unit cells was adequately reproduced during additive manufacturing and the porosity within the struts was minimized. The microstructure of the scaffolds was modified by means of thermal solution and ageing heat treatments and was analysed in detail by means of X-ray microtomography, optical, scanning and transmission electron microscopy. Moreover, the corrosion rates and the mechanical properties of the scaffolds were measured as a function of the strut diameter and metallurgical condition. The microstructure of the as-printed scaffolds contained a mixture of Y-rich oxide particles and Rare Earth-rich intermetallic precipitates. The latter could be modified by heat treatments. The lowest corrosion rates of 2-3 mm/year were found in the as-printed and solution treated scaffolds and they could be reduced to ~0.1 mm/year by surface treatments using plasma electrolytic oxidation. The mechanical properties of the scaffolds improved with the strut diameter: the yield strength increased from 8 to 40 MPa and the elastic modulus improved from 0.2 to 0.8 GPa when the strut diameter increased from 275 \mu m to 800 \mu m. Nevertheless, the strength of the scaffolds without plasma electrolytic oxidation treatment decreased rapidly when immersed in simulated body fluid. In vitro biocompatibility tests showed surface treatments by plasma electrolytic oxidation were necessary to ensure cell proliferation in scaffolds with high surface-to-volume ratio.",2010.03812v1 2020-10-11,Capping layer influence and isotropic in-plane upper critical field of the superconductivity at the FeSe/SrTiO3 interface,"Understanding the superconductivity at the interface of FeSe/SrTiO3 is a problem of great contemporary interest due to the significant increase in critical temperature (Tc) compared to that of bulk FeSe, as well as the possibility of an unconventional pairing mechanism and topological superconductivity. We report a study of the influence of a capping layer on superconductivity in thin films of FeSe grown on SrTiO3 using molecular beam epitaxy. We used in vacuo four-probe electrical resistance measurements and ex situ magneto-transport measurements to examine the effect of three capping layers that provide distinctly different charge transfer into FeSe: compound FeTe, non-metallic Te, and metallic Zr. Our results show that FeTe provides an optimal cap that barely influences the inherent Tc found in pristine FeSe/SrTiO3, while the transfer of holes from a non-metallic Te cap completely suppresses superconductivity and leads to insulating behavior. Finally, we used ex situ magnetoresistance measurements in FeTe-capped FeSe films to extract the angular dependence of the in-plane upper critical magnetic field. Our observations reveal an almost isotropic in-plane upper critical field, providing insight into the symmetry and pairing mechanism of high temperature superconductivity in FeSe.",2010.05308v1 2020-10-16,Synthesis of narrow SnTe nanowires using alloy nanoparticles,"Topological crystalline insulator tin telluride (SnTe) provides a rich playground to examine interactions of correlated electronic states, such as ferroelectricity, topological surface states, and superconductivity. Making SnTe into nanowires further induces novel electronic states due to one-dimensional (1D) confinement effects. Thus, for transport measurements, SnTe nanowires must be made narrow in their diameters to ensure the 1D confinement and phase coherence of the topological surface electrons. This study reports a facile growth method to produce narrow SnTe nanowires with a high yield using alloy nanoparticles as growth catalysts. The average diameter of the SnTe nanowires grown using the alloy nanoparticles is 85 nm, nearly a factor of three reduction from the previous average diameter of 240 nm using gold nanoparticles as growth catalysts. Transport measurements reveal the effect of the nanowire diameter on the residual resistance ratio and magnetoresistance. Particularly, the ferroelectric transition temperature for SnTe is observed to change systematically with the nanowire diameter. In situ cryogenic cooling of narrow SnTe nanowires in a transmission electron microscope directly reveals the cubic to rhombohedral structural transition, which is associated with the ferroelectric transition. Thus, these narrow SnTe nanowires represent a model system to study electronic states arising from the 1D confinement, such as 1D topological superconductivity as well as a potential multi-band superconductivity.",2010.08078v1 2021-02-12,Universal size-dependent nonlinear charge transport in single crystals of the Mott insulator Ca$_2$RuO$_4$,"The surprisingly low current density required for inducing the insulator to metal transition has made Ca$_2$RuO$_4$ an attractive candidate material for developing Mott-based electronics devices. The mechanism driving the resistive switching, however, remains a controversial topic in the field of strongly correlated electron systems. Here we probe an uncovered region of phase space by studying high-purity Ca$_2$RuO$_4$ single crystals, using the sample size as principal tuning parameter. Upon reducing the crystal size, we find a four orders of magnitude increase in the current density required for driving Ca$_2$RuO$_4$ out of the insulating state into a non-equilibrium (also called metastable) phase which is the precursor to the fully metallic phase. By integrating a microscopic platinum thermometer and performing thermal simulations, we gain insight into the local temperature during simultaneous application of current and establish that the size dependence is not a result of Joule heating. The findings suggest an inhomogeneous current distribution in the nominally homogeneous crystal. Our study calls for a reexamination of the interplay between sample size, charge current, and temperature in driving Ca$_2$RuO$_4$ towards the Mott insulator to metal transition.",2102.06556v3 2021-02-23,Huge permittivity and premature metallicity in Bi$_2$O$_2$Se single crystals,"Bi$_2$O$_2$Se is a promising material for next-generation semiconducting electronics. It exhibits premature metallicity on the introduction of a tiny amount of electrons, the physics behind which remains elusive. Here we report on transport and dielectric measurements in Bi$_2$O$_2$Se single crystals at various carrier densities. The temperature-dependent resistivity ($\rho$) indicates a smooth evolution from the semiconducting to the metallic state. The critical concentration for the metal-insulator transition (MIT) to occur is extraordinarily low ($n_\textrm{c}\sim10^{16}$ cm$^{-3}$). The relative permittivity of the insulating sample is huge ($\epsilon_\textrm{r}\approx155(10)$) and varies slowly with temperature. Combined with the light effective mass, a long effective Bohr radius ($a_\textrm{B}^*\approx36(2)$ $\textrm{nm}$) is derived, which provides a reasonable interpretation of the metallic prematurity according to Mott's criterion for MITs. The high electron mobility ($\mu$) at low temperatures may result from the screening of ionized scattering centers due to the huge $\epsilon_\textrm{r}$. Our findings shed light on the electron dynamics in two dimensional (2D) Bi$_2$O$_2$Se devices.",2102.11451v1 2021-04-30,Local inhomogeneities resolved by scanning probe techniques and their impact on local 2DEG formation in oxide heterostructures,"Lateral inhomogeneities in the formation of 2-dimensional electron gases (2DEG) directly influence their electronic properties. Understanding their origin is an important factor for fundamental interpretations, as well as high quality devices. Here, we studied the local formation of the buried 2DEG at LaAlO3/SrTiO3 (LAO/STO) interfaces grown on STO (100) single crystals with partial TiO2 termination, utilizing in-situ local conductivity atomic force microscopy (LC-AFM) and scattering-type scanning near-field optical microscopy (s-SNOM). Using substrates with different degrees of chemical surface termination, we can link the resulting interface chemistry to an inhomogeneous 2DEG formation. In conductivity maps recorded by LC-AFM, a significant lack of conductivity is observed at topographic features, indicative of a local SrO/AlO2 interface stacking order, while significant local conductivity can be probed in regions showing TiO2/LaO interface stacking order. These results could be corroborated by s SNOM, showing a similar contrast distribution in the optical signal which can be linked to the local electronic properties of the material. The results are further complimented by low-temperature conductivity measurements, which show an increasing residual resistance at 5 K with increasing portion of insulating SrO terminated areas. Therefore, we can correlate the macroscopic electrical behavior of our samples to its nanoscopic structure. Using proper parameters, 2DEG mapping can be carried out without any visible alteration of sample properties, proving LC AFM and s SNOM to be viable and destruction-free techniques for the identification of local 2DEG formation. Furthermore, applying LC AFM and s SNOM in this manner opens the exciting prospect to link macroscopic low temperature transport to its nanoscopic origin.",2104.14838v1 2021-05-04,Thermal transport in two-dimensional C3N/C2N superlattices: A molecular dynamics approach,"Nanostructured superlattices have been the focus of many researchers due to their physical and manipulatable properties. They aim to find promising materials for new electronic and thermoelectric devices. In the present study, we investigate the thermal conductivity of two-dimensional (2D) C3N/ C2N superlattices using non-equilibrium molecular dynamics. We analyze the dependence of thermal conductivity on the total length, temperature, and the temperature difference between thermal baths for the superlattices. The minimum thermal conductivity and the phonon mean free path at a superlattice period of 5.2 nm are 23.2W/m.K and 24.7 nm, respectively. Our results show that at a specific total length, as the period increases, the number of interfaces decreases, thus the total thermal resistance decreases, and the effective thermal conductivity of the system increases. We found that at long lengths (L_x >80 nm), the high-frequency and low-wavelength phonons are scattered throughout the interfaces, while at short lengths, there is a wave interference that reduces the thermal conductivity. The combination of these two effects, i.e., the wave interference and the interface scattering, is the reason for the existence of a minimum thermal conductivity in superlattices.",2105.01378v2 2021-07-09,Lithium-Metal Batteries Using Sustainable Electrolyte Media and Various Cathode Chemistries,"Lithium-metal batteries employing concentrated glyme-based electrolytes and different cathode chemistries are herein evaluated in view of a safe use of the highly energetic alkali-metal anode. Indeed, diethylene-glycol dimethyl-ether (DEGDME) and triethylene-glycol dimethyl-ether (TREGDME) dissolving lithium bis(trifluoromethanesulfonyl)imide (LiTFSI) and lithium nitrate (LiNO3) in concentration approaching the solvents saturation limit are used in lithium batteries employing either a conversion sulfur-tin composite (S:Sn 80:20 w/w) or a Li+ (de-)insertion LiFePO4 cathode. Cyclic voltammetry (CV) and electrochemical impedance spectroscopy (EIS) clearly show the suitability of the concentrated electrolytes in terms of process reversibility and low interphase resistance, particularly upon a favorable activation. Galvanostatic measurements performed in the lithium-sulfur (Li/S) batteries reveal promising capacities at room temperature (25 {\deg}C) and a value as high as 1300 mAh gS-1 for DEGDME-based electrolyte at 35 {\deg}C. On the other hand, the lithium-LiFePO4 (Li/LFP) cells exhibit satisfactory cycling behavior, in particular when employing an additional reduction step at low voltage cutoff (i.e., 1.2 V) during the first discharge to consolidate the solid electrolyte interphase (SEI). This procedure allows a coulombic efficiency near 100 %, a capacity approaching 160 mAh g-1 and relevant retention particularly for the cell using TREGDME-based electrolyte. Therefore, this work suggests the use of concentrated glyme-based electrolytes, the fine tuning of the operative conditions, and the careful selection of active materials chemistry as significant steps to achieve practical and safe lithium-metal batteries.",2107.04446v1 2021-08-30,Realization of A Non-Markov Chain in A Single 2D Crystal RRAM,"The non-Markov processes widely exist in thermodymanic processes, while it usually requires packing of many transistors and memories with great system complexity in traditional device architecture to minic such functions. Two-dimensional (2D) material-based resistive random access memory (RRAM) devices show potential for next-generation computing systems with much-reduced complexity. Here, we achieve the non-Markov chain in an individual RRAM device based on 2D mica with a vertical metal/mica/metal structure. We find that the internal potassium ions (K+) in 2D mica gradually move along the direction of the applied electric field, making the initially insulating mica conductive. The accumulation of K+ is tuned by electrical field, and the 2D-mica RRAM possesses both unipolar and bipolar memory windows, high on/off ratio, decent stability and repeatability.Importantly, the non-Markov chain algorithm is established for the first time in a single RRAM, in which the movement of K+ is dependent on the stimulated voltage as well as their past states. This work not only uncovers the inner ionic conductivity of 2D mica, but also opens the door for such novel RRAM devices with numerous functions and applications.",2108.13244v1 2021-09-23,Creating superconductivity in WB2 through pressure-induced metastable planar defects,"High-pressure electrical resistivity measurements reveal that the mechanical deformation of ultra-hard WB2 during compression induces superconductivity above 50 GPa with a maximum superconducting critical temperature, Tc of 17 K at 90 GPa. Upon further compression up to 190 GPa, the Tc gradually decreases. Theoretical calculations show that electron-phonon mediated superconductivity originates from the formation of metastable stacking faults and twin boundaries that exhibit a local structure resembling MgB2} (hP3, space group 191, prototype AlB2). Synchrotron x-ray diffraction measurements up to 145 GPa} show that the ambient pressure hP12 structure (space group 194, prototype WB2) continues to persist to this pressure, consistent with the formation of the planar defects above 50 GPa. The abrupt appearance of superconductivity under pressure does not coincide with a structural transition but instead with the formation and percolation of mechanically-induced stacking faults and twin boundaries. The results identify an alternate route for designing superconducting materials.",2109.11521v2 2021-12-08,Precise Damage Shaping in Self-Sensing Composites Using Electrical Impedance Tomography and Genetic Algorithms,"Fiber-reinforced composites with nanofiller-modified polymer matrices have immense potential to improve the safety of high-risk engineering structures. These materials are intrinsically self-sensing because their electrical conductivity is affected by deformations and damage. This property, known as piezoresistivity, has been extensively leveraged for conductivity-based damage detection via electrical resistance change methods and tomographic imaging techniques such as electrical impedance tomography (EIT). Although these techniques are very effective at detecting the presence of damage, they suffer from an inability to provide precise information about damage shape, size, or mechanism. This is particularly detrimental for laminated composites which can suffer from complex failure modes, such as delaminations, that are difficult to detect. To that end, we herein propose a new technique for precisely determining damage shape and size in self-sensing composites. Our technique makes use of a genetic algorithm (GA) integrated with realistic physics-based damage models to recover precise damage shape from conductivity changes imaged via EIT. We experimentally validate this technique on carbon nanofiber (CNF)-modified glass fiber-reinforced polymer (GFRP) laminates by considering two specific damage mechanisms: through-holes and delaminations. Our results show that this novel technique can accurately reconstruct multiple through-holes with radii as small as 1.19 mm and delaminations caused by low velocity impacts. These findings illustrate that coupling piezoresistivity with conductivity-based spatial imaging techniques and physics-based inversion strategies can enable damage shaping capabilities in self-sensing composite structures.",2112.04419v2 2022-01-10,$B^2$ to $B$-linear magnetoresistance due to impeded orbital motion,"Strange metals exhibit a variety of anomalous magnetotransport properties, the most striking of which is a resistivity that increases linearly with magnetic field $B$ over a broad temperature and field range. The ubiquity of this behavior across a spectrum of correlated metals - both single- and multi-band, with either dominant spin and/or charge fluctuations, of varying levels of disorder or inhomogeneity and in proximity to a quantum critical point or phase - obligates the search for a fundamental underlying principle that is independent of the specifics of any material. Strongly anisotropic (momentum-dependent) scattering can generate $B$-linear magnetoresistance but only at intermediate field strengths. At high enough fields, the magnetoresistance must eventually saturate. Here, we consider the ultimate limit of such anisotropy, a region or regions on the Fermi surface that impede all orbital (cyclotron) motion through them, but whose imposition can be modelled nonetheless through a modified Boltzmann theoretical treatment. Application of the proposed theorem suggests that the realization of quadratic-to-linear magnetoresistance requires the presence of a bounded sector on the Fermi surface possibly separating two distinct types of carriers. While this bounded sector may have different origins or manifestations, we expect its existence to account for the anomalous magnetotransport found in a wide range of correlated materials.",2201.03292v1 2022-01-12,Controlled chemical functionalization toward 3D-2D carbon nanohorn-MoS2 heterostructures with enhanced electrocatalytic activity for protons reduction,"The realization of novel heterostructures arising from the combination of nanomaterials is an effective way to modify their physicochemical and electrocatalytic properties, giving them enhanced characteristics stemming from their individual constituents. Interfacing carbon nanohorns (CNHs) possessing high porosity, large specific surface area and good electrical conductivity, with MoS2 owning multiple electrocatalytic active sites but lacking significant conductivity, robust interactions and effective structure, can be a strategy to boost the electrocatalytic reduction of protons to molecular hydrogen. Herein, we covalently introduce, in a stepwise approach, complementary functional groups at the conical tips and sidewalls of CNHs, along with the basal plane of MoS2, en route the construction of 3D-2D CNH-MoS2 heterostructures. The increased MoS2 loading onto CNHs, improving and facilitating charge delocalization and transfer in neighboring CNHs, along with the plethora of active sites, results in excellent electrocatalytic activity for protons reduction same to that of commercial Pt/C. We have registered minute overpotential, low Tafel slope and small charge-transfer resistance for electrocatalyzing the evolution of hydrogen from the newly prepared heterostructure of 0.029 V, 71 mV/dec and 34.5 {\Omega}, respectively. Furthermore, the stability of the 3D-2D CNH-MoS2 heterostructure was validated after performing 10,000 ongoing electrocatalytic cycles.",2201.05450v1 2022-01-26,AI-Aided Mapping of the Structure-Composition-Conductivity Relationships of Glass-Ceramic Lithium Thiophosphate Electrolytes,"Lithium thiophosphates (LPS) with the composition (Li$_2$S)$_x$(P$_2$S$_5$)$_{1-x}$ are among the most promising prospective electrolyte materials for solid-state batteries (SSBs), owing to their superionic conductivity at room temperature ($>10^{-3}$ S cm$^{-1}$), soft mechanical properties, and low grain boundary resistance. Several glass-ceramic (gc) LPS with different compositions and good Li conductivity have been previously reported, but the relationship between composition, atomic structure, stability, and Li conductivity remains unclear due to the challenges in characterizing non-crystalline phases in experiments or simulations. Here, we mapped the LPS phase diagram by combining first principles and artificial intelligence (AI) methods, integrating density functional theory, artificial neural network potentials, genetic-algorithm sampling, and ab initio molecular dynamics simulations. By means of an unsupervised structure-similarity analysis, the glassy/ceramic phases were correlated with the local structural motifs in the known LPS crystal structures, showing that the energetically most favorable Li environment varies with the composition. Based on the discovered trends in the LPS phase diagram, we propose a candidate solid-state electrolyte composition, (Li$_{2}$S)$_{x}$(P$_{2}$S$_{5}$)$_{1-x}$ ($x\sim{}0.725$), that exhibits high ionic conductivity ($>10^{-2}$ S cm$^{-1}$) in our simulations, thereby demonstrating a general design strategy for amorphous or glassy/ceramic solid electrolytes with enhanced conductivity and stability.",2201.11203v1 2022-03-02,Emergence of insulating ferrimagnetism and perpendicular magnetic anisotropy in 3d-5d perovskite oxide composite films for insulator spintronic,"Magnetic insulators with strong perpendicular magnetic anisotropy (PMA) play a key role in exploring pure spin current phenomena and developing ultralow-dissipation spintronic devices, thereby it is highly desirable to develop new material platforms. Here we report epitaxial growth of La2/3Sr1/3MnO3 (LSMO)-SrIrO3 (SIO) composite oxide films (LSMIO) with different crystalline orientations fabricated by sequential two-target ablation process using pulsed laser deposition. The LSMIO films exhibit high crystalline quality with homogeneous mixture of LSMO and SIO at atomic level. Ferrimagnetic and insulating transport characteristics are observed, with the temperature-dependent electric resistivity well fitted by Mott variable-range-hopping model. Moreover, the LSMIO films show strong PMA. Through further constructing all perovskite oxide heterostructures of the ferrimagnetic insulator LSMIO and a strong spin-orbital coupled SIO layer, pronounced spin Hall magnetoresistance (SMR) and spin Hall-like anomalous Hall effect (SH-AHE) were observed. These results illustrate the potential application of the ferrimagnetic insulator LSMIO in developing all-oxide ultralow-dissipation spintronic devices.",2203.00818v1 2022-04-07,Spin sensitive transport in a spin liquid material: revealing a robustness of spin anisotropy,"Alpha-phase (a-) RuCl_3 has emerged as a prime candidate for a quantum spin liquid (QSL) that promises exotic quasiparticles relevant for fault-tolerant quantum computation. Here, we report spin sensitive transport measurements to probe spin correlation in a-RuCl_3 using a proximal spin Hall metal platinum (Pt). Both transverse and longitudinal resistivities exhibit oscillations as function of the angle between an in-plane magnetic field and the current, akin to previously measured spin Hall magnetoresistance (SMR) in antiferromagnet/Pt heterostructures. The oscillations are observed from 1.5 T to 18 T, both within and beyond the magnetic field range where the antiferromagnetic order and QSL state are reported in a-RuCl_3. The SMR oscillations show that spins in a-RuCl3 are largely locked to an in-plane quantization axis transverse to the magnetic field, constituting a continuous-symmetry-broken state that does not necessarily represent a long-range order. This robust anisotropy of spin axis uncovers critical energy scales connected with reported QSL signatures in a-RuCl_3. Simulations suggest a predominantly antiferromagnetic correlation to moderately high magnetic-fields, that may support the SMR oscillations. The coupling of the spin states within a-RuCl_3 and Pt demonstrated in our experiment opens a transport route to exploring exotic spin phases and device functionalities of QSL materials.",2204.03158v1 2022-06-14,Probing of large interfacial contribution to spin orbit coupling in CoFeB/Ta heterostructure by ultrafast THz emission spectroscopy,"Ultrafast THz radiation generation from ferromagnetic/nonmagnetic bilayer heterostructure-based spintronic emitters generally exploits the conversion from spin- to charge-current within the nonmagnetic layer and its interface with the ferromagnetic layer. Various possible sub-contributions to the underlying mechanism of inverse spin Hall effect for the THz emission from such structures, need to be exploited for not only investigating the intricacies at the fundamental level in the material properties themselves but also for improving their performance for broadband and high-power THz emission. Here, we report ultrafast THz emission from CoFeB/Ta bilayer at varying sample temperatures in a large range to unravel the role of intrinsic and extrinsic spin to charge conversion processes. In addition to an enhancement in the THz emission, its temperature dependence shows a THz signal polarity reversal if the CoFeB/Ta sample is annealed at an elevated temperature. We extract the behaviour of the spin Hall resistivity, determine the intrinsic spin Hall conductivity contribution in it and compare those with the standard Fe/Pt system. Our results clearly demonstrate a giant interfacial contribution to the overall spin Hall angle arising from the modified interface in the annealed CoFeB/Ta, where a sign reversal in the corresponding spin Hall angle is manifested from the THz amplitude variation with the temperature.",2206.06718v2 2022-08-04,Studies on tuning surface electronic properties of hydrogenated diamond by oxygen functionalization,"Ultra-wide bandgap and the absence of shallow dopants are the major challenges in realizing diamond based electronics. However, the surface functionalization offers an excellent alternative to tune electronic structure of diamonds. Herein, we report on tuning the surface electronic properties of hydrogenated polycrystalline diamond films through oxygen functionalization. The hydrogenated diamond (HD) surface transforms from hydrophobic to hydrophilic nature and the sheet resistance increases from ~ 8 kohms/sq. to over 10 Gohms/sq. with progressive ozonation. The conductive atomic force microscopic (c-AFM) studies reveal preferential higher current conduction on selective grain interiors (GIs) than that of grain boundaries confirming the surface charge transfer doping on these HDs. In addition, the local current conduction is also found to be much higher on (111) planes as compared to (100) planes on pristine and marginally O-terminated HD. However, there is no current flow on the fully O-terminated diamond (OD) surface. Further, X-ray photoelectron spectroscopic (XPS) studies reveal a redshift in binding energy (BE) of C1s on pristine and marginally O-terminated HD surfaces indicating surface band bending whilst the BE shifts to higher energy for OD. Moreover, XPS analysis also corroborate c-AFM study for the possible charge transfer doping mechanism on the diamond films which results in high current conduction on GIs of pristine and partially O-terminated HDs.",2208.02465v1 2022-09-01,Four-point bending piezoelectric energy harvester with uniform surface strain toward better energy conversion performance and material usage,"Improving the energy conversion efficiency of piezoelectric energy harvesters is of great importance, and one approach is to make more uniform use of the working material by ensuring a uniform strain state. To achieve better performance, this paper presents a four-point bending piezoelectric energy harvester with extensive investigation and modeling to identify the influential parameters. An electromechanical analytical model is presented and verified by experimental data. The frequency-domain method extracts the solutions for a general time-variable force and impact. Four-point bending is compared with the standard cantilever harvesters regarding voltage generation, mechanical strain, and figure of merit. Strain contours are analyzed and interpreted for this innovative approach, and the power generation by the optimal resistance load is studied. Dimensionless parameters are introduced and investigated to find the optimal operating conditions for the four-point bending harvester. Finally, the four-point bending performance and the best figure of merit are discussed with a view to the long-term fatigue life of the harvester. The results show that in the best four-point bending energy conversion conditions; the energy conversion coefficient is more than three times higher than that of typical cantilever energy harvesters. The results also illustrate that the axial strain experienced in a standard cantilever harvester is more than three times higher than that of the four-point bending harvester, suggesting the latter device may have favorable fatigue performance. Overall, the presented piezoelectric harvester has improved energy conversion efficiency and experiences a reduced and uniform surface strain, making it appropriate for high-efficiency energy harvesting systems.",2209.00252v1 2022-09-08,Observation of strange metal in hole-doped valley-spin insulator,"Temperature-linear resistance at low temperatures in strange metals is an exotic characteristic of strong correlation systems, as observed in high-TC superconducting cuprates, heavy fermions, Fe-based superconductors, ruthenates, and twisted bilayer graphene. Here, we introduce a hole-doped valley-spin insulator, V-doped WSe2, with hole pockets in the valence band. The strange metal characteristic was observed in VxW1-xSe2 at a critical carrier concentration of 9.5 x 10^20 cm-3 from 150 K to 1.8 K. The unsaturated magnetoresistance is almost linearly proportional to the magnetic field. Using the ansatz R(H,T) - R(0,0) ~ [(alpha.k.T)^2+(gamma.mu.B)^2]^1/2, the gamma/alpha ratio is estimated approximately to 4, distinct from that for the quasiparticles of LSCO, BaFe2(As1-xPx)2 (gamma/alpha=1) and bosons of YBCO (gamma/alpha=2). Our observation opens up the possible routes that induce strong correlation and superconductivity in two-dimensional materials with strong spin-orbit coupling.",2209.03672v1 2022-09-26,Study of pnictides for photovoltaic applications,"For the transition into a sustainable mode of energy usage, it is important to develop photovoltaic materials that exhibit better solar-to-electricity conversion efficiencies, a direct optimal band gap, and made of non-toxic, earth abundant elements compared to the state-of-the-art silicon photovoltaics. Here, we explore the non-redox-active pnictide chemical space, including binary A$_3$B$_2$, ternary AA'$_2$B$_2$, and quaternary AA'A""B$_2$ compounds (A, A', A"" = Ca, Sr, or Zn; B = N or P), as candidate beyond-Si photovoltaics using density functional theory calculations. Specifically, we evaluate the ground state configurations, band gaps, and 0 K thermodynamic stability for all 20 pnictide compositions considered, besides computing the formation energy of cation vacancies, anion vacancies, and cation anti-sites in a subset of candidate compounds. Importantly, we identify SrZn$_2$N$_2$, SrZn$_2$P$_2$, and CaZn$_2$P$_2$ to be promising candidates, exhibiting optimal (1.1-1.5 eV) hybrid-functional-calculated band gaps, stability at 0 K, and high resistance to point defects (formation energies $>$1 eV), while other possible candidates include ZnCa$_2$N$_2$ and ZnSr$_2$N$_2$, which may be susceptible to N-vacancy formation. We hope that our study will contribute to the practical development of pnictide semiconductors as beyond-silicon light absorbers.",2209.12458v1 2022-09-28,Dissolution and Recrystallization Behavior of Li3PS4 in Different Organic Solvents,"Solid state batteries can be built based on thiophosphate electrolytes such as beta-Li3PS4. For the preparation of these electrolytes, various solvent-based routes have been reported. For recycling of end-of-life solid state batteries based on such thiophosphates, we consider the development of dissolution and recrystallization strategies for the recovery of the model compound beta-Li3PS4. We show that recrystallization can only be performed in polar, slightly protic solvents such as N-methylformamide (NMF). The recrystallization is comprehensively studied, showing that it proceeds via an intermediate phase with composition Li3PS4*2NMF, which is structurally characterized. This phase has a high resistivity for the transport of lithium ions and must be removed in order to obtain a recrystallized product with a conductivity similar to the pristine material. Moreover, the recrystallization from solution results in an increase of the amorphous phase fraction next to crystalline beta-Li3PS4, which results in a decrease of the activation energy to 0.2 eV compared to 0.38 eV for the pristine phase.",2209.13955v1 2022-11-02,One-Step Formation of Plasmonic Cu Nanodomains in p-Type Cu$_2$O Matrix Films for Enhanced Photoconversion of n-ZnO/p-Cu$_2$O Heterojunctions,"Plasmonic Cu nanoparticles were in-situ grown into a Cu$_2$O semiconductor matrix by using reactive magnetron sputtering and adjusting the amount of oxygen available during the synthesis in order to prevent the oxidation of part of copper atoms landed on the film surface. Varying only the oxygen flowrate (OFR) and using a single Cu target it was possible to observe the evolution in the simultaneous formation of metallic Cu and Cu$_2$O phases for oxygen-poor conditions. Suchformation is accompanied by the development of the surface plasmon band (SPB) corresponding to Cu, as evidenced by UV-Vis spectrophotometry and spectroscopic ellipsometry. The bandgap values of the elaborated composites containing embedded Cu plasmonic nanodomains were lower than the bandgap of single-phased Cu$_2$O films, likely due to the higher defect density associated to the nanocrystalline nature of films, promoted by the presence of metallic Cu. The resistivity of the thin films increased with more oxidative deposition conditions and was associated to an increase in Cu$_2$O/Cu ratio and smaller and more isolated Cu particles, as evidenced by high resolution transmission electron microscopy and X-ray diffraction. Photoconversion devices based on the studied nanocomposites were characterized by I-V and spectral photocurrent measurements, showing an increase in the photocurrent density under light illumination as consequence of the plasmonic particles excitation leading to hot carrier's injection in the nearby ZnO and Cu$_2$O semiconductors.",2211.01010v1 2023-02-25,Strain-adjustable reflectivity of polyurethane nanofiber membrane for thermal management applications,"Passive radiative cooling technologies are highly attractive in pursuing sustainable development. However, current cooling materials are often static, which makes it difficult to cope with the varying needs of all-weather thermal comfort management. Herein, a strategy is designed to obtain flexible thermoplastic polyurethane nanofiber (Es-TPU) membranes via electrospinning, realizing reversible in-situ solvent-free switching between radiative cooling and solar heating through changes in its optical reflectivity by stretching. In its radiative cooling state (0% strain), the Es-TPU membrane shows a high and angular-independent reflectance of 95.6% in the 0.25-2.5 {\mu}m wavelength range and an infrared emissivity of 93.3% in the atmospheric transparency window (8-13 {\mu}m), reaching a temperature drop of 10 {\deg}C at midday, with a corresponding cooling power of 118.25 W/m2. The excellent mechanical properties of the Es-TPU membrane allows the continuous adjustment of reflectivity by reversibly stretching it, reaching a reflectivity of 61.1% ({\Delta}R=34.5%) under an elongation strain of 80%, leading to a net temperature increase of 9.5 {\deg}C above ambient of an absorbing substrate and an equivalent power of 220.34 W/m2 in this solar heating mode. The strong haze, hydrophobicity and outstanding aging resistance exhibited by this scalable membrane hold promise for achieving uniform illumination with tunable strength and efficient thermal management in practical applications.",2302.13043v2 2023-03-26,Molecular lighting goes less powering,"The present era has seen tremendous demands for low-cost electrochromic materials for visible-region multicolor display technology, paper-based, flexible, and wearable electronic devices, smart windows, and optoelectronic applications. Towards this goal, we report large-scale polyelectrochromic devices fabricated on rigid to flexible ITO substrates comprising novel anthracene containing viologen, (1,1'-bis(anthracen-9-ylmethyl)-[4,4'-bipyridine]-1,1'-diium bromide, abbreviated as AnV2+), and polythiophene (P3HT). Inter-estingly, the devices show three states of reversible visible color in response to the applied bias, sub-second to second switching time (0.7 s/1.6 s), and high coloration efficiency (484 cm2/C), longer cycling stability up to 3000 s (103 switching cycles). Thanks to the anthracenes moieties introduced to viologen that inhibit formation of undesired dimer of cation radicals formed in response to the applied bias, other-wise it would hamper the devices reconfiguration. The devices are fully characterized, and electrochromic performances are ensured by bias-dependent UV-Vis, and Raman spectroscopy. The fabricated electro-chromic devices are tested with the commercially available low-cost cells to perform, which is highly de-sired for practical applications. The computational study facilitates the understanding of experimental re-sults. The alternating current (AC)-based electrical impedance spectroscopy reveals that P3HT facilitates reducing charge transfer resistance of the devices. Our work shows CMOS compatibility and one of the best-performing devices that could pave the way for developing cost-effective flexible, and wearable electrochromic devices.",2303.14648v2 2023-04-12,Potential Major Improvement in Superconductors for High-Field Magnets,"Fusion reactors are limited by the magnetic field available to confine their plasma. The commercial fusion industry uses the larger magnetic field and higher operating temperature of the cuprate superconductor $\mathbf{YBa_{2}Cu_{3}O_{7-\delta}}$ (YBCO) in order to confine their plasma into a dense volume. A superconductor is a macroscopic quantum state that is protected from the metallic (resistive) state by an energy gap. Unfortunately, YBCO has an anisotropic gap, known as D-wave because it has the shape of a $\mathbf{d_{x^2-y^2}}$ chemical orbital. This D-wave gap means that poly-crystalline wire cannot be made because a few degree misalignment between grains in the wire leads to a drastic loss in its supercurrent carrying ability, and thereby its magnetic field limit. The superconductor industry has responded by growing nearly-single-crystal superconducting YBCO films on carefully prepared substrate tapes kilometers in length. Heroic development programs have made such tapes commercially available, but they are very expensive and delicate. MRI magnet superconductors, such as $\mathbf{NbTi}$ and $\mathbf{Nb_{3}Sn}$, are formed into poly-crystalline wires because they have an isotropic gap in the shape of an s chemical orbital (called S-wave) that makes them insensitive to grain misalignment. However, these materials are limited to lower magnetic fields and liquid-He temperatures. Here, we modified YBCO by doping the Y site with Ca and Ce atoms to form $\mathbf{(Y_{1-x-y}Ca_{x}Ce_{y})Ba_{2}Cu_{3}O_{7-\delta}}$, and show evidence that it changes to an S-wave gap. Its superconducting transition temperature, $\mathbf{T_c}$, of $\mathbf{\sim 70K}$, while lower than that of D-wave YBCO at $\mathbf{\sim 90K}$, is easily maintained using common, economic cryogenic equipment.",2304.06171v1 2023-05-11,Highly tunable lateral homojunction formed in 2D layered CuInP2S6 via in-plane ionic migration,"As basic building blocks for next-generation information technologies devices, high-quality p-n junctions based on van der Waals (vdW) materials have attracted widespread interest.Compared to traditional two dimensional (2D) heterojunction diodes, the emerging homojunctions are more attractive owing to their intrinsic advantages, such as continuous band alignments and smaller carrier trapping. Here, utilizing the long-range migration of Cu + ions under in-plane electric field, a novel lateral p-n homojunction was constructed in the 2D layered copper indium thiophosphate (CIPS). The symmetric Au/CIPS/Au devices demonstrate an electric-field-driven resistance switching (RS) accompanying by a rectification behavior without any gate control. Moreover, such rectification behavior can be continuously modulated by poling voltage. We deduce that the reversable rectifying RS behavior is governed by the effective lateral build-in potential and the change of the interfacial barrier during the poling process. Furthermore, the CIPS p-n homojuction is evidenced by the photovoltaic effect, with the spectral response extending up to visible region due to the better photogenerated carrier separation efficiency. Our study provides a facile route to fabricate homojuctions through electric-field-driven ionic migration and paves the way towards the use of this method in other vdW materials.",2305.06607v1 2023-06-26,"Spin-flop quasi metamagnetic, anisotropic magnetic, and electrical transport behavior of Ho substituted kagome magnet ErMn$_6$Sn$_6$","We report on the magnetic and electrical properties of a (Mn$_3$Sn)$_2$ triangular network kagome structured high quality Ho substituted ErMn$_6$Sn$_6$ single-crystal sample by magneto-transport measurements. Er$_{0.5}$Ho$_{0.5}$Mn$_6$Sn$_6$ orders antiferromagnetically at N\'{e}el temperature $T_\mathrm{N} \sim$ 350 K followed by a ferrimagnetic (FiM) transition at $T_\mathrm{C} \sim$ 114 K and spin-orientation transition at $T_\mathrm{t} \sim$ 20 K. The field-manifestations of these magnetic phases in the \textit{ab}-basal plane and along the \textit{c}-axis are illustrated through temperature-field \textit{T-H} phase diagrams. In \textit{H}$\parallel$\textit{c}, narrow hysteresis between spin reorientation and field-induced FiM phases below $T_\mathrm{t}$, enhanced/strengthened FiM phase below $T_\mathrm{C}$ and stemming of FiM phase out of strongly coexisting AFM and FiM phases below $T_\mathrm{N}$ through a non-meta-magnetic transition are confirmed to arise from strong R-Mn sublattices interaction. In contrast, \textit{H}$\parallel$\textit{ab}-plane, between $T_\mathrm{N}$ and $T_\mathrm{C}$, individually contributing R-Mn sublattices with weak antiferromagnetic interactions undergo a field-induced spin-flop quasi-metamagnetic transition to FiM state. The temperature dependent electrical resistivity suggests metallic nature with Fermi liquid behavior at low temperatures. Essentially, the current study stimulates interest to investigate the magnetic and electrical properties of mixed rare-earth layered kagome magnetic metals for possible novel and exotic behavior.",2306.14417v1 2023-07-28,Pressure-induced Superconductivity in Zintl Topological Insulator SrIn2As2,"The Zintl compound AIn2X2 (A = Ca, Sr, and X = P, As), as a theoretically predicted new non-magnetic topological insulator, requires experiments to understand their electronic structure and topological characteristics. In this paper, we systematically investigate the crystal structures and electronic properties of the Zintl compound SrIn2As2 under both ambient and high-pressure conditions. Based on systematic angle-resolved photoemission spectroscopy (ARPES) measurements, we observed the topological surface states on its (001) surface as predicted by calculations, indicating that SrIn2As2 is a strong topological insulator. Interestingly, application of pressure effectively tuned the crystal structure and electronic properties of SrIn2As2. Superconductivity is observed in SrIn2As2 for pressure where the temperature dependence of the resistivity changes from a semiconducting-like behavior to that of a metal. The observation of nontrivial topological states and pressure-induced superconductivity in SrIn2As2 provides crucial insights into the relationship between topology and superconductivity, as well as stimulates further studies of superconductivity in topological materials.",2307.15629v1 2023-07-31,Ferroelectricity in tetragonal ZrO$_2$ thin films,"We report on the crystal structure and ferroelectric properties of epitaxial ZrO$_2$ films ranging from 7 to 42 nm thickness grown on La$_{0.67}$Sr$_{0.33}$MnO$_3$-buffered (110)-oriented SrTiO$_3$ substrate. By employing X-ray diffraction, we confirm a tetragonal phase at all investigated thicknesses, with slight in-plane strain due to the substrate in the thinnest films. Further confirmation of the tetragonal phase was obtained through Infrared absorption spectroscopy with synchrotron light, performed on ZrO$_2$ membrane transferred onto a high resistive Silicon substrate. Up to a thickness of 31 nm, the ZrO$_2$ epitaxial films exhibit ferroelectric behavior, at variance with the antiferroelectric behavior reported previously for the tetragonal phase in polycrystalline films. However, the ferroelectricity is found here to diminish with increasing film thickness, with a polarization of about 13 $\mu$C.cm$^{-2}$ and down to 1 $\mu$C.cm$^{-2}$ for 7 nm and 31 nm-thick ZrO$_2$ films, respectively. This highlights the role of thickness reduction, substrate strain, and surface effects in promoting polarization in the tetragonal ZrO$_2$ thin films. These findings provide new insights into the ferroelectric properties and structure of ZrO$_2$ thin films, and open up new directions to investigate the origin of ferroelectricity in ZrO$_2$ and to optimize this material for future applications.",2307.16492v1 2023-08-16,Automated Semiconductor Defect Inspection in Scanning Electron Microscope Images: a Systematic Review,"A growing need exists for efficient and accurate methods for detecting defects in semiconductor materials and devices. These defects can have a detrimental impact on the efficiency of the manufacturing process, because they cause critical failures and wafer-yield limitations. As nodes and patterns get smaller, even high-resolution imaging techniques such as Scanning Electron Microscopy (SEM) produce noisy images due to operating close to sensitivity levels and due to varying physical properties of different underlayers or resist materials. This inherent noise is one of the main challenges for defect inspection. One promising approach is the use of machine learning algorithms, which can be trained to accurately classify and locate defects in semiconductor samples. Recently, convolutional neural networks have proved to be particularly useful in this regard. This systematic review provides a comprehensive overview of the state of automated semiconductor defect inspection on SEM images, including the most recent innovations and developments. 38 publications were selected on this topic, indexed in IEEE Xplore and SPIE databases. For each of these, the application, methodology, dataset, results, limitations and future work were summarized. A comprehensive overview and analysis of their methods is provided. Finally, promising avenues for future work in the field of SEM-based defect inspection are suggested.",2308.08376v2 2023-10-05,Spin-orbit torques and spin Hall magnetoresistance generated by twin-free and amorphous Bi0.9Sb0.1 topological insulator films,"Topological insulators have attracted great interest as generators of spin-orbit torques (SOTs) in spintronic devices. Bi\textsubscript{1-x}Sb\textsubscript{x} is a prominent topological insulator that has a high charge-to-spin conversion efficiency. However, the origin and magnitude of the SOTs induced by current-injection in Bi\textsubscript{1-x}Sb\textsubscript{x} remain controversial. Here we report the investigation of the SOTs and spin Hall magnetoresistance resulting from charge-to-spin conversion in twin-free epitaxial layers of Bi\textsubscript{0.9}Sb\textsubscript{0.1}(0001) coupled to FeCo, and compare it with that of amorphous Bi\textsubscript{0.9}Sb\textsubscript{0.1}. We find a large charge-to-spin conversion efficiency of 1 in the first case and less than 0.1 in the second, confirming crystalline Bi\textsubscript{0.9}Sb\textsubscript{0.1} as a strong spin injector material. The SOTs and spin Hall magnetoresistance are independent of the direction of the electric current, indicating that charge-to-spin conversion in single-crystal Bi\textsubscript{0.9}Sb\textsubscript{0.1}(0001) is isotropic despite the strong anisotropy of the topological surface states. Further, we find that the damping-like SOT has a non-monotonic temperature dependence with a minimum at 20~K. By correlating the SOT with resistivity and weak antilocalization measurements, we conclude that charge-spin conversion occurs via thermally-excited holes from the bulk states above 20~K, and conduction through the isotropic surface states with increasing spin polarization due to decreasing electron-electron scattering below 20~K.",2310.03487v1 2023-12-09,Extended Kohler's Rule of Magnetoresistance in TaCo$_2$Te$_2$,"TaCo$_2$Te$_2$ is recently reported to be an air-stable, high mobility Van der Waals material with probable magnetic order. Here we investigate the scaling behavior of its magnetoresistance. We measured both the longitudinal ($\rho_{xx}$) and Hall ($\rho_{xy}$) magnetoresistivities of TaCo$_2$Te$_2$ crystals in magnetic fields parallel to the c-axis and found that the magnetoresistance violates the Kohler's rule $MR \sim f[H/\rho_0]$ while obeying the extended Kohler's rule $MR \sim f[H/(n_T\rho_0)]$, where $MR \sim [\rho_{xx}(H)-\rho_0]/\rho_0$, $H$ is the magnetic field, $n_T$ is a thermal factor, $\rho_{xx}(H)$ and $\rho_0$ are the resistivities at $H$ and zero field, respectively. While deviating from those of the densities of electrons ($n_e$) and holes ($n_h$) obtained from the two-band model analysis of the magnetoconductivities, the temperature dependence of $n_T$ is close to that of the Hall carrier densities $n_H$ calculated from the slopes of $\rho_{xy}(H)$ curves at low magnetic fields, providing a new way to obtain the thermal factor in the extended Kohler's rule.",2312.05624v1 2023-12-16,"Electronic phase transition, vibrational properties and structural stability of single and two polyyne chains under external electric field","Search for one dimensional (1D) van der Waals materials has become an urgent need to meet the demand as building blocks for high performance, miniaturized, lightweight device applications. Polyyne, a 1D atomic chain of carbon is the thinnest and strongest allotrope of carbon, showing promising applications in new generation low dimensional devices due to the presence of a band gap. A system of two carbon chains held together by van der Waals interaction has been theoretically postulated and shows band gap tunability under structural changes which finds applications in the realms of resistive switching and spintronics. In this study, we use first principles Density Functional Theory (DFT) to show a sharp semiconductor to metal transition along with the emergence of an asymmetry in the spin polarized density of states for single and two polyyne chains under a transverse electric field. The thermodynamic stability of the system has been substantiated through the utilization of Ab Initio Molecular Dynamics (AIMD) simulations, phonon dispersion curve analyses, and formation energy calculations. Furthermore, in addition to its dynamic stability assessment, phonon calculations have served to identify Raman active vibrational modes which offers an invaluable non-destructive experimental avenue for discerning electronic phase transitions in response to an applied electric field. Our study presents a predictive framework for the prospective utilization of one and two polyyne chains in forthcoming flexible nano-electronic and spintronic devices. The future prospects of the system are contingent upon advancements in nano-electronics fabrication techniques and the precise construction of circuitry for harnessing spin-related applications.",2312.10335v1 2024-02-06,Observation of the double quantum spin Hall phase in moiré WSe2,"Quantum spin Hall (QSH) insulators are a topologically protected phase of matter in two dimensions that can support non-dissipative spin transport. A hallmark of the phase is a pair of helical edge states surrounding an insulating bulk. A higher (even) number of helical edge state pairs is usually not possible in real materials because spin mixing would gap out the edge states. Multiple pairs of helical edge states have been proposed in materials with spin conservation symmetry and high spin Chern bands, but remained experimentally elusive. Here, we demonstrate a QSH phase with one and two pairs of helical edge states in twisted bilayer WSe2 at moir\'e hole filling factor {\nu}= 2 and 4, respectively. We observe nearly quantized conductance or resistance plateaus of h/({\nu}e^2 ) at {\nu} = 2 and 4 while the bulk is insulating. The conductance is nearly independent of out-of-plane magnetic field and decreases under an in-plane magnetic field. We also observe nonlocal transport, which is sensitive only to the in-plane magnetic field. The results agree with quantum transport of helical edge states protected by Ising spin conservation symmetry and open a promising platform for low-power spintronics.",2402.04196v1 2024-02-13,Coarse-Graining in Space versus Time,"Understanding the structure and dynamics of liquids is pivotal for the study of larger spatiotemporal processes, particularly for glass-forming materials at low temperatures. The so-called thermodynamic scaling relation, validated for many molecular systems through experiments, offers an efficient means to explore a vast range of time scales along a one-dimensional phase diagram. Isomorph theory provides a theoretical framework for thermodynamic scaling based on strong virial-potential energy correlations, but this approach is most successful for simple point particles. In particular, isomorph theory has resisted extension to complex molecular liquids due to the existence of high-frequency intramolecular interactions. To elucidate the microscopic origin of density scaling for molecular systems, we employ two distinct approaches for coarse-graining in space or in time. The former eliminates fast degrees of freedom by reducing a molecule to a center-of-mass-level description, while the latter involves temporally averaged fluctuations or correlation functions over the characteristic time scale. We show that both approaches yield a consistent density scaling coefficient for ortho-terphenyl, which is moreover in agreement with the experimental value. Building upon these findings, we derive the density scaling relationship exhibiting a single-parameter phase diagram from fully atomistic simulations. Our results unravel the microscopic nature underlying thermodynamic scaling and shed light on the role of coarse-graining for assessing the slow fluctuations in molecular systems, ultimately enabling the extension of systematic bottom-up approaches to larger and more complex molecular liquids that are experimentally challenging to probe.",2402.08675v1 2024-02-27,Design principles of nonlinear optical materials for Terahertz lasers,"We have investigated both inter-band and intra-band second order nonlinear optical conductivity based on the velocity correlation formalism and the spectral expansion technique. We propose a scenario in which the second order intra-band process is nonzero while the inter-band process is zero. This occurs for a band structure with momentum asymmetry in the Brillouin zone. Very low-energy photons are blocked by the Pauli exclusion principle from participating in the inter-band process; however, they are permitted to participate in the intra-band process, with the band smeared by some impurity scattering. We establish a connection between the inter-band nonlinear optical conductivity in the velocity gauge and the shift vector in the length gauge for a two-band model. Using a quasiclassical kinetic approach, we demonstrate the importance of intra-band transitions in high harmonic generations for the single tilted Dirac cone model and hexagonal warping model. We confirm that the Kramers-Kronig relations break down for the limit case of ($\omega$, $-\omega$) in the nonlinear optical conductivity. Finally, we calculate the superconducting transition temperature of NbN and the dielectric function of AlN, and the resistance of the NbN/AlN junction. The natural non-linearity of the Josephson junction brings a Josephson plasma with frequency in the Terahertz region.",2402.17126v1 2024-03-25,Multi-Objective Quality-Diversity for Crystal Structure Prediction,"Crystal structures are indispensable across various domains, from batteries to solar cells, and extensive research has been dedicated to predicting their properties based on their atomic configurations. However, prevailing Crystal Structure Prediction methods focus on identifying the most stable solutions that lie at the global minimum of the energy function. This approach overlooks other potentially interesting materials that lie in neighbouring local minima and have different material properties such as conductivity or resistance to deformation. By contrast, Quality-Diversity algorithms provide a promising avenue for Crystal Structure Prediction as they aim to find a collection of high-performing solutions that have diverse characteristics. However, it may also be valuable to optimise for the stability of crystal structures alongside other objectives such as magnetism or thermoelectric efficiency. Therefore, in this work, we harness the power of Multi-Objective Quality-Diversity algorithms in order to find crystal structures which have diverse features and achieve different trade-offs of objectives. We analyse our approach on 5 crystal systems and demonstrate that it is not only able to re-discover known real-life structures, but also find promising new ones. Moreover, we propose a method for illuminating the objective space to gain an understanding of what trade-offs can be achieved.",2403.17164v1 2002-08-26,Magnetized Accretion-Ejection Structures: 2.5D MHD simulations of continuous Ideal Jet launching from resistive accretion disks,"We present numerical magnetohydrodynamic (MHD) simulations of a magnetized accretion disk launching trans-Alfvenic jets. These simulations, performed in a 2.5 dimensional time-dependent polytropic resistive MHD framework, model a resistive accretion disk threaded by an initial vertical magnetic field. The resistivity is only important inside the disk, and is prescribed as eta = alpha_m V_AH exp(-2Z^2/H^2), where V_A stands for Alfven speed, H is the disk scale height and the coefficient alpha_m is smaller than unity. By performing the simulations over several tens of dynamical disk timescales, we show that the launching of a collimated outflow occurs self-consistently and the ejection of matter is continuous and quasi-stationary. These are the first ever simulations of resistive accretion disks launching non-transient ideal MHD jets. Roughly 15% of accreted mass is persistently ejected. This outflow is safely characterized as a jet since the flow becomes super-fastmagnetosonic, well-collimated and reaches a quasi-stationary state. We present a complete illustration and explanation of the `accretion-ejection' mechanism that leads to jet formation from a magnetized accretion disk. In particular, the magnetic torque inside the disk brakes the matter azimuthally and allows for accretion, while it is responsible for an effective magneto-centrifugal acceleration in the jet. As such, the magnetic field channels the disk angular momentum and powers the jet acceleration and collimation. The jet originates from the inner disk region where equipartition between thermal and magnetic forces is achieved. A hollow, super-fastmagnetosonic shell of dense material is the natural outcome of the inwards advection of a primordial field.",0208459v1 2006-02-17,Coupling losses and transverse resistivity of multifilament YBCO coated superconductors,"We studied the magnetization losses of four different types of filamentary YBCO coated conductors. A 10 mm wide YBCO coated conductor was subdivided into 20 filaments by laser cutting. The separation of coupling loss from the total is possible because the energy loss per cycle in samples with electrically insulated filaments has a very small frequency dependence. We measured the frequency dependence of the total losses in the frequency range between 0.1 Hz and 500 Hz. The coupling loss was obtained from the total by subtracting the hysteresis loss. The latter was measured at low frequencies since only hysteresis loss is non-negligible at frequencies below 1 Hz. The transverse resistivity was determined from the coupling losses; it was assumed that the sample length is equal to half of the twist pitch. The values of transverse resistivity deduced from the loss data were compared with those obtained by the four-point measurements with current flowing perpendicular to the filaments. Preliminary results indicate that the current method of laser ablation creates electrical contacts between the superconducting filaments and the substrate. This was also confirmed by the Hall probe mapping of the magnetic field in the vicinity of the tape. The measured transverse resistivity was close to the resistivity of the substrate (Hastelloy).",0602422v1 2007-02-21,Electrical current-driven pinhole formation and insulator-metal transition in tunnel junctions,"Current Induced Resistance Switching (CIS) was recently observed in thin tunnel junctions (TJs) with ferromagnetic (FM) electrodes and attributed to electromigration of metallic atoms in nanoconstrictions in the insulating barrier. The CIS effect is here studied in TJs with two thin (20 \AA) non-magnetic (NM) Ta electrodes inserted above and below the insulating barrier. We observe resistance (R) switching for positive applied electrical current (flowing from the bottom to the top lead), characterized by a continuous resistance decrease and associated with current-driven displacement of metallic ions from the bottom electrode into the barrier (thin barrier state). For negative currents, displaced ions return into their initial positions in the electrode and the electrical resistance gradually increases (thick barrier state). We measured the temperature (T) dependence of the electrical resistance of both thin- and thick-barrier states ($R_b$ and R$_B$ respectively). Experiments showed a weaker R(T) variation when the tunnel junction is in the $R_b$ state, associated with a smaller tunnel contribution. By applying large enough electrical currents we induced large irreversible R-decreases in the studied TJs, associated with barrier degradation. We then monitored the evolution of the R(T) dependence for different stages of barrier degradation. In particular, we observed a smooth transition from tunnel- to metallic-dominated transport. The initial degradation-stages are related to irreversible barrier thickness decreases (without the formation of pinholes). Only for later barrier degradation stages do we have the appearance of metallic paths between the two electrodes that, however, do not lead to metallic dominated transport for small enough pinhole radius.",0702501v2 2008-12-15,Nanomechanical detection of antibiotic-mucopeptide binding in a model for superbug drug resistance,"The alarming growth of the antibiotic-resistant superbugs methicillin-resistant Staphylococcus aureus (MRSA) and vancomycin-resistant Enterococcus (VRE) is driving the development of new technologies to investigate antibiotics and their modes of action. We report the label-free detection of vancomycin binding to bacterial cell wall precursor analogues (mucopeptides) on cantilever arrays, with 10 nM sensitivity and at clinically relevant concentrations in blood serum. Differential measurements quantified binding constants for vancomycin-sensitive and vancomycin-resistant mucopeptide analogues. Moreover, by systematically modifying the mucopeptide density we gain new insights into the origin of surface stress. We propose that stress is a product of a local chemical binding factor and a geometrical factor describing the mechanical connectivity of regions affected by local binding in terms of a percolation process. Our findings place BioMEMS devices in a new class of percolative systems. The percolation concept will underpin the design of devices and coatings to significantly lower the drug detection limit and may also impact on our understanding of antibiotic drug action in bacteria.",0812.2728v1 2010-05-19,Resistance in Superconductors,"In this pedagogical review, we discuss how electrical resistance can arise in superconductors. Starting with the idea of the superconducting order parameter as a condensate wave function, we introduce vortices as topological excitations with quantized phase winding, and we show how phase slips occur when vortices cross the sample. Superconductors exhibit non-zero electrical resistance under circumstances where phase slips occur at a finite rate. For one-dimensional superconductors or Josephson junctions, phase slips can occur at isolated points in space-time. Phase slip rates may be controlled by thermal activation over a free-energy barrier, or in some circumstances, at low temperatures, by quantum tunneling through a barrier. We present an overview of several phenomena involving vortices that have direct implications for the electrical resistance of superconductors, including the Berezinskii-Kosterlitz-Thouless transition for vortex-proliferation in thin films, and the effects of vortex pinning in bulk type II superconductors on the non-linear resistivity of these materials in an applied magnetic field. We discuss how quantum fluctuations can cause phase slips and review the non-trivial role of dissipation on such fluctuations. We present a basic picture of the superconductor-to-insulator quantum phase transitions in films, wires, and Josephson junctions. We point out related problems in superfluid helium films and systems of ultra-cold trapped atoms. While our emphasis is on theoretical concepts, we also briefly describe experimental results, and we underline some of the open questions.",1005.3347v1 2013-06-28,Impact of sintering temperature on room temperature magneto-resistive and magneto-caloric properties of Pr2/3Sr1/3MnO3,"Magneto-resistive and magneto-caloric properties of polycrystalline Pr2/3Sr1/3MnO3 have been studied as a function of sintering temperature (Ts) between 1260-1450{\deg}C. Reitveld refinement of their X-ray diffraction (XRD) patterns confirms their single phase crystalline structure with orthorhombic Pbnm space group. The point of maximum value of temperature coefficient of resistance (TCRmax) and Curie temperature (Tc) decreased slightly with Ts. Magneto-resistance (MR) and magnetic entropy ({\Delta}SM) increased markedly with sintering temperature. This could be attributed to the observed sharpness of both the magnetic and resistive transitions due to better grain connectivity. Optimum results are obtained for the sample with Ts = 1400{\deg}C. MR at Tc of the same is found to be as large as 32% at 1T and 58% at 5T magnetic fields. The maximum entropy change ({\Delta}SMmax) near its Tc is 2.3Jkg-1K-1 and 7.8 Jkg-1K-1 upon 1T and 5T fields change respectively. These characteristics [MR (32% 1T, 58% 5T) and reasonable change in magnetic entropy (7.8Jkg-1K-1, 5T)] generate possibility that the optimized compound can be used as a potential magnetic refrigerant close to room temperature.",1306.6792v2 2014-11-15,Shock-waves and commutation speed of memristors,"Progress of silicon based technology is nearing its physical limit, as minimum feature size of components is reaching a mere 10 nm. The resistive switching behaviour of transition metal oxides and the associated memristor device is emerging as a competitive technology for next generation electronics. Significant progress has already been made in the past decade and devices are beginning to hit the market; however, it has been mainly the result of empirical trial and error. Hence, gaining theoretical insight is of essence. In the present work we report the striking result of a connection between the resistive switching and {\em shock wave} formation, a classic topic of non-linear dynamics. We argue that the profile of oxygen vacancies that migrate during the commutation forms a shock wave that propagates through a highly resistive region of the device. We validate the scenario by means of model simulations and experiments in a manganese-oxide based memristor device. The shock wave scenario brings unprecedented physical insight and enables to rationalize the process of oxygen-vacancy-driven resistive change with direct implications for a key technological aspect -- the commutation speed.",1411.4198v3 2015-09-29,Extraordinary Hall resistance and unconventional magnetoresistance in Pt/LaCoO3 hybrids,"We report an investigation of transverse Hall resistance and longitudinal resistance on Pt thin films sputtered on epitaxial LaCoO$_3$ (LCO) ferromagnetic insulator films. The LaCoO$_3$ films were deposited on several single crystalline substrates [LaAlO$_3$ (LAO), (La,Sr)(Al,Ta)O$_3$ (LSAT), and SrTiO$_3$ (STO)] with (001) orientation. The physical properties of LaCoO$_3$ films were characterized by the measurements of magnetic and transport properties. The LaCoO$_3$ films undergo a paramagnetic to ferromagnetic (FM) transition at Curie temperatures ranging from 40 K to 85 K, below which the Pt/LCO hybrids exhibit significant extraordinary Hall resistance (EHR) up to 50 m$\Omega$ and unconventional magnetoresistance (UCMR) ratio $\Delta$$\rho$/$\rho_0$ about $1.2 \times 10^{-4}$, accompanied by the conventional magnetoresistance (CMR). The observed spin transport properties share some common features as well as some unique characteristics when compared with well-studied Y$_3$Fe$_5$O$_{12}$-based Pt thin films. Our findings call for new theories since the extraordinary Hall resistance and magnetoresistance cannot be consistently explained by the existing theories.",1509.08691v1 2016-02-24,Contact resistances in trigate and FinFET devices in a Non-Equilibrium Green's Functions approach,"We compute the contact resistances $R_{\rm c}$ in trigate and FinFET devices with widths and heights in the 4 to 24 nm range using a Non-Equilibrium Green's Functions approach. Electron-phonon, surface roughness and Coulomb scattering are taken into account. We show that $R_{\rm c}$ represents a significant part of the total resistance of devices with sub-30 nm gate lengths. The analysis of the quasi-Fermi level profile reveals that the spacers between the heavily doped source/drain and the gate are major contributors to the contact resistance. The conductance is indeed limited by the poor electrostatic control over the carrier density under the spacers. We then disentangle the ballistic and diffusive components of $R_{\rm c}$, and analyze the impact of different design parameters (cross section and doping profile in the contacts) on the electrical performances of the devices. The contact resistance and variability rapidly increase when the cross sectional area of the channel goes below $\simeq 50$ nm$^2$. We also highlight the role of the charges trapped at the interface between silicon and the spacer material.",1602.07545v1 2017-10-26,Effect of air confinement on thermal contact resistance in nanoscale heat transfer,"We report herein the pressure dependent thermal contact resistance (Rc) between Wollaston wire thermal probe and samples which is evaluated within the framework of an analytical model. This work presents heat transfer between the Wollaston wire thermal probe and samples at nanoscale for different air pressure ranging from 1 Pa to 10e5 Pa. We make use of a scanning thermal microscopy (SThM) for the thermal analysis of two samples, fused silica (SiO2) and Titanium (Ti), with different thermal conductivities. The thermal probe's output voltage difference (deltaV) between out-off contact output voltage (Voc) and in-contact output voltage (Vic) was recorded. The result shows that the heat transfer increases with the increasing air pressure and it is found higher for higher thermal conductive material. We also propose an analytical model based on the normalized output voltage difference to extract the probe-sample thermal contact resistance. The obtained Rc values in the range of ~1.8e7 K/W to ~14.3e7 K/W validate the presented analytical model. Further analysis reveals that the thermal contact resistance between the probe and sample decreases with increasing air pressure. Such behavior is interpreted by the contribution of heat transfer through confined air on thermal contact resistance. In addition, the signature of Rc is also evidenced in the context of thermal mismatch behavior which is studied by using acoustic mismatch model (AMM) and diffuse mismatch model (DMM).",1710.09501v1 2017-11-08,Surface impedance and optimum surface resistance of a superconductor with imperfect surface,"We calculate a low-frequency surface impedance of a dirty, s-wave superconductor with an imperfect surface incorporating either a thin layer with a reduced pairing constant or a thin, proximity-coupled normal layer. Such structures model realistic surfaces of superconducting materials which can contain oxide layers, absorbed impurities or nonstoichiometric composition. We solved the Usadel equations self-consistently and obtained spatial distributions of the order parameter and the quasiparticle density of states which then were used to calculate a low-frequency surface resistance $R_s(T)$ and the magnetic penetration depth $\lambda(T)$ as functions of temperature in the limit of local London electrodynamics. It is shown that the imperfect surface in a single-band s-wave superconductor results in a non-exponential temperature dependence of $Z(T)$ at $T\ll T_c$ which can mimic the behavior of multiband or d-wave superconductors. The imperfect surface and the broadening of the gap peaks in the quasiparticle density of states $N(\epsilon)$ in the bulk give rise to a weakly temperature-dependent residual surface resistance. We show that the surface resistance can be optimized and even reduced below its value for an ideal surface by engineering $N(\epsilon)$ at the surface using pairbreaking mechanisms, particularly, by incorporating a small density of magnetic impurities or by tuning the thickness and conductivity of the normal layer and its contact resistance. The results of this work address the limit of $R_s$ in superconductors at $T\ll T_c$, and the ways of engineering the optimal density of states by surface nano-structuring and impurities to reduce losses in superconducting micro-resonators, thin film strip lines, and radio frequency cavities for particle accelerators.",1711.03077v1 2018-02-15,Parallel magnetic field suppresses dissipation in superconducting nanostrips,"The motion of Abrikosov vortices in type-II superconductors results in a finite resistance in the presence of an applied electric current. Elimination or reduction of the resistance via immobilization of vortices is the ""holy grail"" of superconductivity research. Common wisdom dictates that an increase in the magnetic field escalates the loss of energy since the number of vortices increases. Here we show that this is no longer true if the magnetic field and the current are applied parallel to each other.Our experimental studies on the resistive behavior of a superconducting Mo$_{0.79}$Ge$_{0.21}$ nanostrip reveal the emergence of a dissipative state with increasing magnetic field, followed by a pronounced resistance drop, signifying a reentrance to the superconducting state. Large-scale simulations of the 3D time-dependent Ginzburg-Landau model indicate that the intermediate resistive state is due to an unwinding of twisted vortices. When the magnetic field increases, this instability is suppressed due to a better accommodation of the vortex lattice to the pinning configuration. Our findings show that magnetic field and geometrical confinement can suppress the dissipation induced by vortex motion and thus radically improve the performance of superconducting materials.",1802.05673v1 2018-05-22,Structural properties and anisotropic electronic transport in SrIrO3 films,"Perovskite SrIrO3 (SIO) films epitaxially deposited with a thickness of about 60 nm on various substrate materials display nearly strain-relieved state. Films grown on orthorhombic (110) DyScO3 (DSO) are found to display untwinned bulk-like orthorhombic structure. However, film deposition on cubic (001) SrTiO3 induces a twinned growth of SIO. Resistance measurements on the SIO films reveal only weak temperature dependence, where the resistance R increases with decreasing temperature T. Hall measurements show dominant electron-like transport throughout the temperature range from 2 K to 300 K. At 2 K, the electron concentration and resistivity for SIO on STO amount to ne = 1.4*10^20 cm-3 and 1 mohmcm. Interestingly, the film resistance of untwinned SIO on DSO along the [1-10] and the [001] direction differs by up to 25% indicating pronounced anisotropic electronic transport. The anisotropy of the resistance increases with decreasing T and displays a distinct maximum around 86 K. The specific T-dependence is similar to that of the structural anisotropy sqrt(a2+b2)/c of bulk SIO. Therefore, anisotropic electronic transport in SIO is very likely induced by the orthorhombic distortion. Consequently, for twinned SIO films on STO anisotropy vanishes nearly completely. The experimental results show that structural changes are very likely responsible for the observed anisotropic electronic transport. The strong sensitivity of the electronic transport in SIO films may be explained in terms of the narrow electron-like bands in SIO caused by spin-orbit-coupling and orthorhombic distortion.",1805.08473v2 2022-02-24,Thermal spreading resistance of GaN HEMTs with heat source heating studied by hybrid Monte Carlo-diffusion simulations,"Exact assessment of thermal spreading resistance is of great importance to the thermal management of electronic devices, especially when completely considering the heat conduction process from the nanoscale heat source to the macroscopic scale heat sink. The existing simulation methods are either based on convectional Fourier's law or limited to small system sizes, making it difficult to accurately and efficiently study the cross-scale heat transfer. In this paper, a hybrid phonon Monte Carlo-diffusion method that couples phonon Monte Carlo (MC) method with Fourier's law by dividing the computational domain is adopted to analyze thermal spreading resistance in ballistic-diffusive regime. Compared with phonon MC simulation, the junction temperature of the hybrid method has the same precision, while the time costs could be reduced up to 2 orders of magnitude at most. Furthermore, the simulation results indicate that the heating scheme has a remarkable impact on phonon transport. The thermal resistance of the heat source (HS) scheme can be larger than that of the heat flux (HF) scheme, which is opposite from the prediction of Fourier's law. In the HS scheme, the enhanced phonon-boundary scattering counteracts the broadening of the heat source, leading to a stronger ballistic effect as the heat source thickness decreases. The conclusion is verified by a one-dimensional thermal resistance model. This work has opened up an opportunity for the fast and extensive thermal modeling of cross-scale heat transfer in electronic devices and highlighted the influence of heating schemes.",2202.13770v1 2007-10-10,Strong Reduction of the Field-Dependent Microwave Surface Resistance in YBCO with BaZrO_3 Inclusions,"We present measurements of the magnetic field dependent microwave surface resistance in laser-ablated YBa$_2$Cu$_3$O$_{7-\delta}$ films on SrTiO$_3$ substrates. BaZrO$_3$ crystallites were included in the films using composite targets containing BaZrO$_3$ inclusions with mean grain size smaller than 1 $\mu$m. X-ray diffraction showed single epitaxial relationship between BaZrO$_3$ and YBa$_2$Cu$_3$O$_{7-\delta}$. The effective surface resistance was measured at 47.7 GHz for 60$< T <$90 K and 0$< \mu_0H <$0.8 T. The magnetic field had a very different effect on pristine YBa$_2$Cu$_3$O$_{7-\delta}$ and YBa$_2$Cu$_3$O$_{7-\delta}$/BaZrO$_3$, while for $\mu_0H=$0 only a reduction of $T_c$ in the YBa$_2$Cu$_3$O$_{7-\delta}$/BaZrO$_3$ film was observed, consistent with dc measurements. At low enough $T$, in moderate fields YBa$_2$Cu$_3$O$_{7-\delta}$/BaZrO$_3$ exhibited an intrinsic thin film resistance lower than the pure film. The results clearly indicate that BaZrO$_3$ inclusions determine a strong reduction of the field-dependent surface resistance. From the analysis of the data in the framework of simple models for the microwave surface impedance in the mixed state we argue that BaZrO$_3$ inclusions determine very steep pinning potentials.",0710.1953v1 2018-07-19,Theoretical study of scattering in graphene ribbons in the presence of structural and atomistic edge roughness,"We investigate the diffusive electron-transport properties of charge-doped graphene ribbons and nanoribbons with imperfect edges. We consider different regimes of edge scattering, ranging from wide graphene ribbons with (partially) diffusive edge scattering to ribbons with large width variations and nanoribbons with atomistic edge roughness. For the latter, we introduce an approach based on pseudopotentials, allowing for an atomistic treatment of the band structure and the scattering potential, on the self-consistent solution of the Boltzmann transport equation within the relaxation-time approximation and taking into account the edge-roughness properties and statistics. The resulting resistivity depends strongly on the ribbon orientation, with zigzag (armchair) ribbons showing the smallest (largest) resistivity and intermediate ribbon orientations exhibiting intermediate resistivity values. The results also show clear resistivity peaks, corresponding to peaks in the density of states due to the confinement-induced subband quantization, except for armchair-edge ribbons that show a very strong width dependence because of their claromatic behavior. Furthermore, we identify a strong interplay between the relative position of the two valleys of graphene along the transport direction, the correlation profile of the atomistic edge roughness, and the chiral valley modes, leading to a peculiar strongly suppressed resistivity regime, most pronounced for the zigzag orientation.",1807.07263v2 2020-10-07,Correlation of uniaxial magnetic anisotropy axes and principal resistivities in polycrystalline ferromagnetic films,"In the present study, we demonstrate the measurement of resistivity tensor ($\rho$) along the magnetic axes of a polycrystalline film of ferromagnetic permalloy (Py). To this end, conventional Hall-bar and a more recent extended van der Pauw methods were utilized for determining 2D $\rho$ in the film plane. The samples were prepared by normal incidence sputter deposition within an in-situ magnetic field to induce in-plane uniaxial magnetic anisotropy in the film. Since $\rho$ might be affected by the internal magnetization of the film, we performed measurements by rotation of a saturating magnetic field in the film plane. Both methods indicate that the average resistivity is lower along the easy axis of the film compared to the hard axis. Since X-ray diffraction results indicated no dominating texture in the film, we concluded that there is a correlation between uniaxial magnetic axes and principal resistivity axes. This is an important finding that allows determining the direction of magnetic anisotropy axes without magnetometry. The results also verify atomic or pair ordering to be the origin of uniaxial magnetic anisotropy in the Py since resistivity is sensitive to the level of order in solids. The extended van der Pauw utilized here can be easily performed on the as-received samples which is of practical interest.",2010.03554v3 2020-12-31,DC Resistance Degradation of SrTiO$_3$: The Role of Virtual-Cathode Needles and Oxygen Bubbles,"This study of highly accelerated lifetime tests of SrTiO$_3$, a model semiconducting oxide, is motivated by the interest in reliable multilayer ceramic capacitors and resistance-switching thin-film devices. Our analytical solution to oxygen-vacancy migration under a DC voltage -- the cause of resistance degradation in SrTiO$_3$ -- agrees with previous numerical solutions. However, all solutions fail to explain why degradation kinetics feature a very strong voltage dependence, which we attribute to the nucleation and growth of cathode-initiated fast-conducting needles. While they have no color contrast in SrTiO$_3$ single crystals and are nominally invisible, needles presence in DC-degraded samples -- in silicone oil and in air -- was unambiguously revealed by in-situ hot-stage photography. Observations in silicone oil and thermodynamic considerations of voltage boundary conditions further revealed a cooccurrence of copious oxygen bubbling and the onset of final accelerating degradation, suggesting sudden oxygen loss is a precursor of final failure. Remarkably, both undoped and Fe-doped SrTiO$_3$ can emit electroluminescence at higher current densities, thus providing a vivid indicator of resistance degradation and a metal-to-insulator resistance transition during cooling. The implications of these findings to thin ceramic and thin film SrTiO$_3$ devices are discussed, along with connections to similar findings in likewise degraded fast-ion yttria-stabilized zirconia.",2012.15777v1 2021-04-12,Temperature-linear Resistivity in Twisted Double Bilayer Graphene,"We report an experimental study of carrier density (n), displacement field (D) and twist angle ({\theta}) dependence of temperature (T)-linear resistivity in twisted double bilayer graphene (TDBG). For a large twist angle ({\theta}>1.5{\deg}) where correlated insulating states are absent, we observe a T-linear resistivity (with the slope of the order ~10{\Omega}/K) over a wide range of carrier density and its slope decreases with increasing of n, in agreement with acoustic phonon scattering model semi-quantitatively. The slope of T-linear resistivity is non-monotonically dependent on the displacement field with a single peak structure. For device with {\theta}~1.23{\deg} at which correlated states emerge, the slope of T-linear resistivity is found maximum (~100{\Omega}/K) at the boundary of the halo structure where phase transition occurs, with signatures of continuous phase transition, Planckian dissipation, and the diverging effective mass; these observations are in line with quantum critical behaviors, which might be due to the symmetry-breaking instability at the critical points. Our results shed new light on correlated physics in TDBG and other twisted moir\'e systems.",2104.05406v3 2022-01-06,Coulomb drag in metal monochalcogenides double-layer structures with Mexican-hat band dispersions,"We theoretically study the Coulomb drag resistivity and plasmon modes behavior for a system composed of two parallel p-type doped GaS monolayers with Mexican-hat valence energy band using the Boltzmann transport theory formalism. We investigate the effect of temperature,$\ T$, carrier density,$\ p$, and layer separation,$\ d$, on the plasmon modes and drag resistivity within the energy-independent scattering time approximation. Our results show that the density dependence of plasmon modes can be approximated by$\ p^{0.5}$. Also, the calculations suggest a$\ d^{0.2}$ and a$\ d^{0.1}$ dependencies for the acoustic and optical plasmon energies, respectively. Interestingly, we obtain that the behavior of drag resistivity in the double-layer metal monochalcogenides swings between the behavior of a double-quantum well system with parabolic dispersion and that of a double-quantum wire structure with a large carrier density of states. In particular, the transresistivity value reduces exponentially with increasing the distance between layers. Furthermore, the drag resistivity changes as$\ T^{2}/p^{4}$ ($\ T^{2.8}/p^{4.5}$) at low (intermediate) temperatures. Finally, we compare the drag resistivity as a function of temperature for GaS with other Mexican-hat materials including GaSe and InSe and find that it adopts higher values when the metal monochalcogenide has smaller Mexican-hat height.",2201.02077v1 2023-02-14,Acoustic phonon contribution to the resistivity of twisted bilayer graphene,"We calculate the contribution to the doping ($n$) and temperature ($T$) dependence of the electrical resistivity of twisted bilayer graphene (TBLG) due to scattering by acoustic phonons. Our calculation retains the full Bistritzer-MacDonald (BM) band structure, with a focus on understanding the role of the complicated geometric features present in the BM band structure on electronic transport theory. We find that the band geometry plays an important role in determining the resistivity, giving an intricate dependence on both $n$ and $T$ that mirrors features in the band structure and complicates the Bloch-Gr\""{u}neisen (BG) crossover. Our calculations predict pronounced departures from the standard simplistic expectation of a linear $T$-dependence above the BG crossover. In particular, we are able to explain the presence of the resistance peaks that have been observed in experiment, as well as quantitatively predict the temperatures at which they occur. Our calculated theoretical results are germane to an ongoing debate over the existence of a strange metal state in TBLG by providing a quantitatively accurate theory for the TBLG resistivity at finite temperatures.",2302.07275v3 2023-04-21,Star-Mesh Quantized Hall Array Resistance Devices,"Advances in the development of graphene-based technology have enabled improvements in DC resistance metrology. Devices made from epitaxially grown graphene have replaced the GaAs-based counterparts, leading to an easier and more accessible realization of the ohm. By optimizing the scale of the growth, it has become possible to fabricate quantized Hall array resistance standards (QHARS) with nominal values between 1 k{\Omega} and 1.29 M{\Omega}. One of these QHARS device designs accommodates a value of about 1.01 M{\Omega}, which made it an ideal candidate to pursue a proof-of-concept that graphene-based QHARS devices are suitable for forming wye-delta resistance networks. In this work, the 1.01 M{\Omega} array output nearly 20.6 M{\Omega} due to the wye-delta transformation, which itself is a special case of star-mesh transformations. These mathematical equivalence principles allow one to extend the QHR to the 100 M{\Omega} and 10 G{\Omega} resistance levels with fewer array elements than would be necessary for a single array with many more elements in series. The 1.01 M{\Omega} device shows promise that the wye-delta transformation can shorten the calibration chain, and, more importantly, provide a chain with a more direct line to the quantum SI.",2304.11243v1 2023-06-12,"Symmetric, off-diagonal, resistance from rotational symmetry breaking in graphene-WSe$_2$ heterostructure: prediction for a large magic angle in a Moire system","We show that any two-dimensional system with a non-zero \textit{symmetric} off-diagonal component of the resistance matrix, $R_{xy}=R_{yx} \neq 0$, must have the in-plane rotational symmetry broken down to $C_2$. Such a resistance response is Ohmic, and is different from the Hall response which is the \textit{anti-symmetric} part of the resistance tensor, $R_{xy}=-R_{yx}$, is rotationally symmetric in the 2D plane, and requires broken time-reversal symmetry. We show how a minute amount of strain due to lattice mismatch - less than $1 \%$ - can produce a vastly exaggerated symmetric off-diagonal response - $\frac{R_{xy}}{R_{xx}} \sim 20\%$ - because of the momentum matching constraints in a Moire system. Our results help explain an important new transport experiment on graphene-WSe$_2$ heterostructures, as well as are relevant for other experimental systems with rotational symmetry breaking, such as nematic systems and Kagome charge density waves. Additionally, our work predicts an example of a `magic' angle, $\theta\sim 27^0$, in a Moire system which is a significant fraction of $\pi$. Our prediction that the anomalous resistance anisotropy occurs at a large value of magic angle, in contrast to known examples of magic angle transport anomalies that are small fractions of $\pi$, can be experimentally tested in graphene-WSe$_2$ heterostructures.",2306.06840v2 2024-03-04,"Electric field induced resistive switching in M$^{3+}_x$V$_{1-x}$O$_2$ (M$^{3+}$= Ga$^{3+}$, Al$^{3+}$) single crystals at temperatures below the T $\to$ M2 phase transition","The phase diagram of VO$_2$ strained or doped with several trivalent ions consists of four phases; in order of increasing temperatures, three (M1, T and M2) are insulating while the fourth (R), above ~340 K, is metallic. These phases and the three phase transitions have been thoroughly investigated for about half a century by a wide variety of techniques, including electronic transport. While an upwards jump of the resistance of up to a factor of 2 was observed at the T-M2 transition and a drop of several orders of magnitude was observed at the M2$\to$R one, resistive switching at the M1$\to$T transition remained elusive over all these years. Here we report on the investigation of Ga- and Al-doped VO$_2$ single crystals, following the rather surprising appearance of a small and steep drop of a factor of ~ 0.12 in the resistance of Ga-doped VO$_2$ single crystals detected by pulsed and DC I-V measurements carried out at room temperature, below the T$\to$M2 phase transition. Similar results were obtained also from measurements on Al-doped VO2 single crystals. Raman spectra of Ga-, and Al-doped crystals resolved their structures as function of temperature. The accumulated results of the measurements on Ga-, and Al-doped single crystals provide evidence for identifying the resistive switching at T$_{\rm RS}$0.5*10^11 cm^-2, the resistivity increases with increasing T and is linear above 50K, suggesting carrier scattering from acoustic phonons. At T=240K the mobility is ~120,000 cm^2/Vs, higher than in any known semiconductor. At the charge neutral point we observe a non-universal conductivity that decreases with decreasing T, consistent with a density inhomogeneity <10^8 cm^-2.",0805.1830v1 2008-06-20,Effective Resistance Mismatch and Magnetoresistance of a CPP-GMR system with Current-Confined-Paths,"We theoretically study the magnetoresistance of a CPP-GMR system with current confined paths (CCP) in the framework of Valet-Fert theory. The continuity equations for charge and spin currents are numerically solved with the three-dimensional CCP geometry by use of finite element method. It is confirmed that the MR ratio is enhanced by the CCP structure, which is consistent with the experimental results. Moreover, we find that there exists a certain contact width which maximize the MR ratio. We show that the contact width which maximize the MR ratio is well described by the effective resistance matching.",0806.3314v1 2008-06-26,Negative differential resistance in molecular junctions: The effect of the electrodes electronic structure,"We have carried out calculations of electron transport through a metal-molecule-metal junction with metal nanoclusters taking the part of electrodes. We show that negative differential resistance peaks could appear in the current-voltage curves. The peaks arise due to narrow features in the electron density of states of the metal clusters. The proposed analysis is based on the ab initio computations of the relevant wave functions and energies within the framework of the density functional theory using NRLMOL software package.",0806.4397v2 2008-10-07,Huge anisotropic magneto-resistance in iridium atomic chains,"We analyze in this article the magneto-resistance ratio of finite and infinite iridium and platinum chains. Our calculations, that are based on a combination of non equilibrium Green function techniques and density functional theory, include a fully self-consistent treatment of non-collinear magnetism and of the spin-orbit interaction. They indicate that, in addition to having an extremely large magnetic anisotropy that may overcome the super-paramagnetic limit, infinite and also realistic finite-length iridium chains show sizeable anisotropic magnetoresistance ratios. We therefore propose iridium nanostructures as promising candidates for nanospintronics logic devices.",0810.1170v1 2008-10-22,Itinerant Ferromagnetism in the electronic localization limit,"We present Hall effect, $R_{xy}(H)$, and magnetoresistance, $R_{xx}(H)$, measurements of ultrathin films of Ni, Co and Fe with thicknesses varying between 0.2-8 nm and resistances between 1 M$\Omega$ - 100 $\Omega.$ Both measurements show that films having resistance above a critical value, $R_{C}$, (thickness below a critical value, $d_{C}$) show no signs for ferromagnetism. Ferromagnetism appears only for films with $R in the limit v->0 is not zero owing to the mutual collisions between the intervening particles. The nonzero F_0 implies the appearance of kinetic friction in this simple dynamical system.",0909.2132v1 2009-10-13,Superconductivity of FeSe0.5Te0.5 Thin Films Grown by Pulsed Laser Deposition,"FeSe0.5Te0.5 thin films with PbO-type structure are successfully grown on MgO(100) and LaSrAlO4(001) substrates from FeSe0.5Te0.5 or FeSe0.5Te0.75 polycrystalline targets by pulsed-laser deposition. The film deposited on the MgO substrate (film thickness ~ 55 nm) shows superconductivity at 10.6 K (onset) and 9.2 K (zero resistivity). On the other hand, the film deposited on the LaSrAlO4 substrate (film thickness ~ 250 nm) exhibits superconductivity at 5.4 K (onset) and 2.7 K (zero resistivity). This suggests the strong influence of substrate materials and/or the c-axis length to superconducting properties of FeSe0.5Te0.5 thin films.",0910.2301v1 2010-01-25,Evidence for effective thermal boundary resistance from magnon/phonon disequilibrium,"We use the time-resolved magneto-optical Kerr effect (TRMOKE) to measure the local temperature and heat flow dynamics in ferromagnetic SrRuO3 thin films. After heating by a pump pulse, the film temperature decays exponentially, indicating that the heat flow out of the film is limited by the film/substrate interface. We show that this behavior is consistent with an effective boundary resistance resulting from disequilibrium between the spin and phonon temperatures in the film.",1001.4557v1 2010-03-12,Electronic phase diagram of NdFe1-xRhxAsO,"We report on the electrical resistivity, thermoelectric power and electronic phase diagram of rhodium-doped NdFeAsO. Rhodium doping suppresses the structural phase transition and spin density wave observed in the undoped material, and superconductivity emerges at x close to 0.05, despite the distortion of FeAs4 tetrahedra induced by the large size difference between Rh and Fe elements. The Tc(x) curve is dome-like, and the highest Tc is reached at x = 0.1, with Tconset = 18K. An upturn of the electrical resistivity above Tc has been observed, with a Kondo like behaviour above Tc and a Fermi-liquid behaviour close to room temperature.",1003.2528v1 2010-06-02,Emergence of current branches in a series array of negative differential resistance circuit elements,"We study a series array of nonlinear electrical circuit elements that possess negative differential resistance and find that \emph{heterogeneity} in the element properties leads to the presence of multiple branches in current-voltage curves and a non-uniform distribution of voltages across the elements. An inhomogeneity parameter $r_{max}$ is introduced to characterize the extent to which the individual element voltages deviate from one another, and it is found to be strongly dependent on the rate of change of applied voltage. Analytical expressions are derived for the dependence of $r_{max}$ on voltage ramping rate in the limit of fast ramping and are confirmed by direct numerical simulation.",1006.0434v1 2010-10-08,On giant piezoresistance effects in silicon nanowires and microwires,"The giant piezoresistance (PZR) previously reported in silicon nanowires is experimentally investigated in a large number of surface depleted silicon nano- and micro-structures. The resistance is shown to vary strongly with time due to electron and hole trapping at the sample surfaces. Importantly, this time varying resistance manifests itself as an apparent giant PZR identical to that reported elsewhere. By modulating the applied stress in time, the true PZR of the structures is found to be comparable with that of bulk silicon.",1010.1633v1 2011-03-08,Electric--field effect on electron-doped infinite-layer Sr$_{0.88}$La$_{0.12}$CuO$_{2+x}$ thin films,"We have used the electric--field effect to modulate the resistivity of the surface of underdoped Sr$_{0.88}$La$_{0.12}$CuO$_{2+x}$ thin films, allowing opposite modifications of the electron and hole density in the CuO$_2$ planes, an original situation with respect to conventional chemical doping in electron-doped materials. When the Hall effect indicates a large contribution of a hole band, the electric--field effect on the normal state resistivity is however dominated by the electrons, and the superconducting transition temperature increases when carriers are transfered from holes to electrons.",1103.1548v2 2011-03-17,Structure-related transport properties of A-site ordered perovskite Sr3ErMn4-xGaxO10.5-d,"We report x-ray diffraction, resistivity, thermopower, and magnetization of Sr3ErMn4-xGaxO10.5-d, in which A-site ordered tetragonal phase appears above x=1, and reveal that the system exhibits typical properties seen in the antiferromagnetic insulator with Mn3+. We succeed in preparing both A-site ordered and disordered phases for x=1 in different preparation conditions, and observe a significant decrease of the resistivity in the disordered phase. We discuss possible origins of the decrease focusing on the dimensionality and the disordered effect.",1103.3342v1 2011-08-19,"Hydrostatic pressure study of paramagnetic-ferromagnetic phase transition in (Ga,Mn)As","The effect of hydrostatic pressure on the paramagnetic - ferromagnetic phase transition has been studied in (Ga,Mn)As. The variation of the Curie temperature (TC) with pressure was monitored by two transport methods: (1) - measurement of zero field resistivity versus temperature {\rho}(T), (2) - dependence on temperature of the Hall voltage hysteresis loop. Two specimens of different resistivity characteristics were examined. The measured pressure-induced changes of TC were relatively small (of the order of 1K/GPa) for both samples, however they were opposite for the two.",1108.3960v1 2011-09-26,Anomalous Hall effect in the Co-based Heusler compounds Co$_{2}$FeSi and Co$_{2}$FeAl,"The anomalous Hall effect (AHE) in the Heusler compounds Co$_{2}$FeSi and Co$_{2}$FeAl is studied in dependence of the annealing temperature to achieve a general comprehension of its origin. We have demonstrated that the crystal quality affected by annealing processes is a significant control parameter to tune the electrical resistivity $\rho_{xx}$ as well as the anomalous Hall resistivity $\rho_{ahe}$. Analyzing the scaling behavior of $\rho_{ahe}$ in terms of $\rho_{xx}$ points to a temperature-dependent skew scattering as the dominant mechanism in both Heusler compounds.",1109.5498v1 2011-10-22,Anomalous negative differential thermal resistance in a momentum-conserving lattice,"A two-segment Fermi-Pasta-Ulam lattices has been investigated by using nonequilibrium molecular dynamics. Here we present an anomalous negative differential thermal resistance (NDTR) that have not been reported in Frenkel-Kontorova and \phi_4 lattices up to the present. The NDTR disappears at low temperature region. The region of NDTR shifts from the large to the small temperature difference region as the system size increases. Anomalous dependence of NDTR on the temperature can be explained as the negative effect induced by the nonlinear coupling. The explanation can also cover the phenomenon of NDTR in momentum-nonconserved lattices.",1110.4942v1 2011-12-09,Temperature Coefficient of Resistivity in Amorphous Semiconductors,"By invoking the microscopic response method in conjunction with a reasonable set of approximations, we obtain new explicit expressions for the electrical conductivity and temperature coefficient of resistivity (TCR) in amorphous semiconductors, especially a-Si:H and a-Ge:H. The predicted TCR for n-doped a-Si:H and a-Ge:H is in agreement with experiments. The conductivity from the transitions from a localized state to an extended state (LE) is comparable to that from the transitions between two localized states (LL). This resolves a long-standing anomaly, a ""kink"" in the experimental $\log_{10}\sigma $ vs. T$^{-1}$ curve.",1112.2169v2 2012-08-19,Interplay between sheet resistance increase and magnetotransport properties in ${\rm LaAlO_3}/{\rm SrTiO_3}$,"We find that the sheet resistance ($R_s$) of patterned samples of ${\rm LaAlO_3}/{\rm SrTiO_3}$ with a length scale of several microns may increase significantly at low temperatures in connection with driving electrical currents and applying in-plane magnetic fields. As the samples are warmed up, $R_s$ recovers to its original value with accelerated recovery near ${\rm 70 \ K}$ and ${\rm 160 \ K}$. Concomitantly with the increase in $R_s$, the carrier density and the mobility decrease and magnetotransport properties which may be linked to magnetism are suppressed.",1208.3837v1 2012-09-24,Observation of linear-polarization-sensitivity in the microwave-radiation-induced magnetoresistance oscillations,"In the quasi two-dimensional GaAs/AlGaAs system, we investigate the effect of rotating \textit{in-situ} the electric field of linearly polarized microwaves relative to the current, on the microwave-radiation-induced magneto-resistance oscillations. We find that the frequency and the phase of the photo-excited magneto-resistance oscillations are insensitive to the polarization. On the other hand, the amplitudes of the magnetoresistance oscillations are remarkably responsive to the relative orientation between the microwave antenna and the current-axis in the specimen. The results suggest a striking linear-polarization-sensitivity in the radiation-induced magnetoresistance oscillations.",1209.5135v1 2012-10-09,Thermopower as sensitive probe of electronic nematicity in iron pnictides,"We study the in-plane anisotropy of the thermoelectric power and electrical resistivity on detwinned single crystals of isovalent substituted EuFe$_{2}$(As$_{1-x}$P$_{x}$)$_2$. Compared to the resistivity anisotropy the thermopower anisotropy is more pronounced and clearly visible already at temperatures much above the structural and magnetic phase transitions. Most remarkably, the thermopower anisotropy changes sign below the structural transition. This is associated with the interplay of two contributions due to anisotropic scattering and orbital polarization, which dominate at high- and low-temperatures, respectively.",1210.2634v2 2012-10-29,Anomalous Energy Transport across Topological Insulator Superconductor Junctions,"We study the nonequilibrium energy transport across a topological insulator/superconductor junction, by deriving an interfacial heat current formula through scattering wave approach. Several anomalous thermal properties are uncovered, such as thermal energy's Klein tunneling, asymmetric Kapitza resistance and negative differential thermal resistance. We expect these findings could have potential applications for the energy control in various hybridized mesoscopic systems.",1210.7551v2 2012-10-29,Resistance Switching Induced by Electric Field and Light Illumination in Device of FTO/CeO2/Electrolyte/FTO,"A heterojunction-like device consisting of FTO/CeO2/electrolyte/FTO is established with distinct transport performance, where FTO denotes F-doped transparent conducting glass, and the electrolyte is LiI and I2 in acetonitrile. The resistive switching behavior is observed, being induced through applying sufficient negative pulse as well as light illumination. The endurance measurements confirm that the write/erase periodic operation is reproducible and stable in the present device. Furthermore, the retention measurements demonstrate that the information can be stored temporarily for about 100 seconds. A possible mechanism regarding the formation of diiodide radical is proposed to give a reasonable explanation for the observed switching behavior.",1210.7558v2 2012-11-06,Angular dependence of the Hall effect of lsmo films,"We find that the Hall effect resistivity ($\rho_{xy}$) of thin films of \lsmo\ varies as a function of the angle $\theta$ between the applied magnetic field and the film normal as $\rho_{xy}=a\cos \theta + b\cos 3\theta$, where $|b|$ increases with increasing temperature and decreases with increasing magnetic field. We find that the angular dependence of the longitudinal resistivity and the magnetization cannot fully explain the surprising term $b$, suggesting it is a manifestation of an intrinsic transport property.",1211.1160v1 2013-09-25,Magnetic and transport properties of Mn2CoAl oriented thin films,"The structure, magnetic and transport properties of thin films of the Heusler ferrimagnet Mn_{2}CoAl have been investigated for properties related to spin gapless semiconductors. Oriented films were grown by molecular beam epitaxy on GaAs substrates and the structure was found to transform from tetragonal to cubic for increasing annealing temperature. The anomalous Hall resistivity is found to be proportional to the square of the longitudinal resistivity and magnetization expected for a topological Berry curvature origin. A delicate balance of the spin-polarized carrier type when coupled with voltage gate-tuning could significantly impact advanced electronic devices.",1309.6660v1 2014-02-15,Ferromagnetism and transport properties of the Kondo system Ce4Sb1.5Ge1.5,"Ferromagnetic ordering with a small magnetic moment is found below 14 K from SQUID measurements for the compound Ce4Sb1.5Ge1.5. The transport characteristics of a number of Ce4Sb3-xTx (T = Ge, Si, Sn, Pb, Al) systems were measured at room temperature, Ce4Sb1.5Ge1.5 demonstrating the highest Seebeck coefficient. Its transport properties (resistivity, thermal conductivity, thermoelectric power) are experimentally investigated in detail up to low temperatures. The Kondo-lattice behavior of resistivity and its anomaly at the ordering point are found. A comparison with the Wiedemann-Franz law is performed.",1402.3667v2 2014-02-20,Transverse ultrasonic anomaly in La1/3Sr2/3MnO3,"The charge ordering (CO) transition in polycrystalline La1/3Sr2/3MnO3 has been studied by measuring the resistivity, magnetization and transverse ultrasonic velocity. At about 235K, a conspicuous increase in resistivity was observed, while the magnetization shows a cusp structure, corresponding to an antiferromagnetic charge ordering transition. Around this transition temperature, dramatic anomaly in transverse sound velocity was observed. The simultaneous occurrence of electron, magnon and phonon anomalous features implies strong spin-phonon coupling and electron-phonon in La1/3Sr2/3MnO3. The analysis suggests that the spin-phonon interaction is due to single-ion magnetostriction, and electron-phonon coupling originates from the Jahn-Teller effect of Mn3+.",1402.4857v2 2014-03-01,Anomalies of transport properties in antiferromagnetic YbMn2Sb2 compound,"The low-temperature transport properties (resistivity, thermal conductivity, thermoelectric power) are experimentally investigated for the compound YbMn2Sb2. Large Seebeck coefficient and nearly linear temperature dependence of resistivity are obtained. The thermal conductivity is large and has mainly phonon origin. Appreciable anomalies of transport characteristics near the antiferromagnetic transition point are found. Possible influence of pseudo-Kondo scattering is discussed.",1403.0077v2 2014-05-23,Photovoltaic performance of n-type SnS active layer in ITO/PEDOT:PSS/SnS/Al structure,"The present paper discusses the influence of Tin Sulphide's grain size on the performance of ITO/PEDOT:PSS/SnS/Al structured solar cells fabricated by thermal evaporation. The grain sizes were maintained in the range of 11-18~nm by controlling the thickness of SnS films. While the open circuit voltage (Voc) was found to be a constant for this structure, Parameters such as short circuit current density (Jsc), series resistance (Rs), parallel resistance (Rp), ideality factor and the overall efficiency were found to be dependent on the SnS grain size and incident light intensity. The experimental work directly reconfirms the theoretical results and ideas raised in literature by early researchers.",1405.6013v1 2014-07-29,Proximity coupling of granular film with ferroelectric substrate and giant electro-resistance effect,"We study electron transport in granular film placed above the ferroelectric substrate. We show that the conductivity of granular film strongly depends on the ferroelectric state due to screening effects which modify the Coulomb blockade in granular film. In particular, the electric current in granular film is controlled by the direction of ferroelectric polarization. We show that the ferroelectric/granular film system has a large electro-resistance effect. This effect can be utilized in memory and electric field sensor applications.",1407.7719v2 2014-10-28,Tunable Solid State and Flexible Graphene Electronics,"We demonstrate tunable solid state and flexible graphene field effect devices (FEDs) fabricated using a poly(methylmethacrylate) (PMMA) and lithium fluoride (LiF) composite dielectric. Increasing the concentration of LiF in the composite dielectric reduces the operating gate voltages significantly from 10 V to 1 V required leading to a decrease in resistance. Electron and hole mobility of 350 and 310 cm2/Vs at VD = -5 V are obtained for graphene FEDs with 10 % LiF concentration in the composite. Using composite dielectric also enabled excellent performance on flexible substrates without any significant change in mobility and resistance. Flexible FEDs with only 5 % and 12 % variation in mobility for 300 and 750 bending are obtained.",1410.7563v1 2015-12-29,Scaling like behaviour of resistivity observed in LaNiO_3 thin films grown on SrTiO_3 substrate by pulsed laser deposition,"We discuss the origin of the temperature dependence of resistivity observed in highly oriented LaNiO_3 thin films (of thickness d) grown on SrTiO_3 substrate by a pulsed laser deposition technique. All the experimental data are found to collapse into a single universal curve [T/T_{sf}(d)]^{3/2} for the entire temperature interval (20K20) are challenging, due to the low thermal resistance of the thin film compared to that of the substrate. In principle, {\Lambda}_cross could be measured by time-domain thermoreflectance (TDTR), using a high modulation frequency f_h and a large laser spot size. However, with one TDTR measurement at f_h, the uncertainty of the TDTR measurement is usually high due to low sensitivity of TDTR signals to {\Lambda}_cross and high sensitivity to the thickness h_Al of Al transducer deposited on the sample for TDTR measurements. We observe that in most TDTR measurements, the sensitivity to h_Al only depends weakly on the modulation frequency f. Thus, we performed an additional TDTR measurement at a low modulation frequency f_0, such that the sensitivity to h_Al is comparable but the sensitivity to {\Lambda}cross is near zero. We then analyze the ratio of the TDTR signals at f_h to that at f_0, and thus significantly improve the accuracy of our {\Lambda}cross measurements. As a demonstration of the dual-frequency approach, we measured the cross-plane thermal conductivity of a 400-nm-thick nickel-iron alloy film and a 3-{\mu}m-thick Cu film, both with an accuracy of ~10%. The dual-frequency TDTR approach is useful for future studies of thin films.",1511.04852v2 2015-12-04,2D layered transport properties from topological insulator Bi$_2$Se$_3$ single crystals and micro flakes,"Low-field magnetotransport measurements of topological insulators such as Bi$_2$Se$_3$ are important for revealing the nature of topological surface states by quantum corrections to the conductivity, such as weak-antilocalization. Recently, a rich variety of high-field magnetotransport properties in the regime of high electron densities ($\sim10^{19}$ cm$^{-3}$) were reported, which can be related to additional two-dimensional layered conductivity, hampering the identification of the topological surface states. Here, we report that quantum corrections to the electronic conduction are dominated by the surface states for a semiconducting case, which can be analyzed by the Hikami-Larkin-Nagaoka model for two coupled surfaces in the case of strong spin-orbit interaction. However, in the metallic-like case this analysis fails and additional two-dimensional contributions need to be accounted for. Shubnikov-de Haas oscillations and quantized Hall resistance prove as strong indications for the two-dimensional layered metallic behavior. Temperature-dependent magnetotransport properties of high-quality Bi$_2$Se$_3$ single crystalline exfoliated macro and micro flakes are combined with high resolution transmission electron microscopy and energy-dispersive x-ray spectroscopy, confirming the structure and stoichiometry. Angle-resolved photoemission spectroscopy proves a single-Dirac-cone surface state and a well-defined bulk band gap in topological insulating state. Spatially resolved core-level photoelectron microscopy demonstrates the surface stability.",1512.01442v2 2015-12-22,Dome-shaped magnetic order competing with high-temperature superconductivity at high pressures in FeSe,"The coexistence and competition between superconductivity and electronic orders, such as spin or charge density waves, have been a central issue in high transition-temperature (${T_{\rm c}}$) superconductors. Unlike other iron-based superconductors, FeSe exhibits nematic ordering without magnetism whose relationship with its superconductivity remains unclear. More importantly, a pressure-induced fourfold increase of ${T_{\rm c}}$ has been reported, which poses a profound mystery. Here we report high-pressure magnetotransport measurements in FeSe up to $\sim9$ GPa, which uncover a hidden magnetic dome superseding the nematic order. Above ${\sim6}$ GPa the sudden enhancement of superconductivity (${T_{\rm c}\le38.3}$ K) accompanies a suppression of magnetic order, demonstrating their competing nature with very similar energy scales. Above the magnetic dome we find anomalous transport properties suggesting a possible pseudogap formation, whereas linear-in-temperature resistivity is observed above the high-${T_{\rm c}}$ phase. The obtained phase diagram highlights unique features among iron-based superconductors, but bears some resemblance to that of high-${T_{\rm c}}$ cuprates.",1512.06951v1 2016-06-06,Comeback of epitaxial graphene for electronics: large-area growth of bilayer-free graphene on SiC,"We present a new fabrication method for epitaxial graphene on SiC which enables the growth of ultra-smooth defect- and bilayer-free graphene sheets with an unprecedented reproducibility, a necessary prerequisite for wafer-scale fabrication of high quality graphene-based electronic devices. The inherent but unfavorable formation of high SiC surface terrace steps during high temperature sublimation growth is suppressed by rapid formation of the graphene buffer layer which stabilizes the SiC surface. The enhanced nucleation is enforced by decomposition of polymer adsorbates which act as a carbon source. With most of the steps well below 0.75 nm pure monolayer graphene without bilayer inclusions is formed with lateral dimensions only limited by the size of the substrate. This makes the polymer assisted sublimation growth technique the most promising method for commercial wafer scale epitaxial graphene fabrication. The extraordinary electronic quality is evidenced by quantum resistance metrology at 4.2 K with until now unreached precision and high electron mobilities on mm scale devices.",1606.01709v1 2018-06-01,Amplifier for scanning tunneling microscopy at MHz frequencies,"Conventional scanning tunneling microscopy (STM) is limited to a bandwidth of circa 1kHz around DC. Here, we develop, build and test a novel amplifier circuit capable of measuring the tunneling current in the MHz regime while simultaneously performing conventional STM measurements. This is achieved with an amplifier circuit including a LC tank with a quality factor exceeding 600 and a home-built, low-noise high electron mobility transistor (HEMT). The amplifier circuit functions while simultaneously scanning with atomic resolution in the tunneling regime, i.e. at junction resistances in the range of giga-ohms, and down towards point contact spectroscopy. To enable high signal-to-noise and meet all technical requirements for the inclusion in a commercial low temperature, ultra-high vacuum STM, we use superconducting cross-wound inductors and choose materials and circuit elements with low heat load. We demonstrate the high performance of the amplifier by spatially mapping the Poissonian noise of tunneling electrons on an atomically clean Au(111) surface. We also show differential conductance spectroscopy measurements at 3MHz, demonstrating superior performance over conventional spectroscopy techniques. Further, our technology could be used to perform impedance matched spin resonance and distinguish Majorana modes from more conventional edge states.",1806.00374v1 2019-09-27,Distinctive Thermoelectric Properties of Supersaturated Si-Ge-P Compounds: Achieving Figure of Merit ZT > 3.6,"The efficiency of energy conversion in thermoelectric generators (TEGs) is directly proportional to electrical conductivity and Seebeck coefficient while inversely to thermal conductivity. The challenge is to optimize these interdependent parameters simultaneously. In this work, the problem is addressed with a novel approach of nanostructuring and constructive electronic structure modification to achieve a very high value of dimensionless figure of merit ZT greater than 3.6 at 1000 K with negative Seebeck coefficient. Supersaturated solid-solutions of Si-Ge containing 1 atomic percent Fe and 10 atomic percent P are prepared by high-energy ball milling. The bulk samples consisting of ultra-fine nano-crystallites 9.7 nm are obtained by the sophisticated low-temperature & high-pressure sintering process. Despite that the electrical resistivity is slightly high due to the localization of electrons is associated with the highly disordered structure and low electrical density of states near the chemical potential, a very low thermal conductivity \k{appa} less than 1 W m-1K-1 and very large magnitude of Seebeck coefficient exceeding 470 uV K-1 are achieved in association with the nanostructuring and the Fe 3d impurity states, respectively, to realize a very large magnitude of ZT.",1909.12476v1 2019-02-27,Learning nonlinear level sets for dimensionality reduction in function approximation,"We developed a Nonlinear Level-set Learning (NLL) method for dimensionality reduction in high-dimensional function approximation with small data. This work is motivated by a variety of design tasks in real-world engineering applications, where practitioners would replace their computationally intensive physical models (e.g., high-resolution fluid simulators) with fast-to-evaluate predictive machine learning models, so as to accelerate the engineering design processes. There are two major challenges in constructing such predictive models: (a) high-dimensional inputs (e.g., many independent design parameters) and (b) small training data, generated by running extremely time-consuming simulations. Thus, reducing the input dimension is critical to alleviate the over-fitting issue caused by data insufficiency. Existing methods, including sliced inverse regression and active subspace approaches, reduce the input dimension by learning a linear coordinate transformation; our main contribution is to extend the transformation approach to a nonlinear regime. Specifically, we exploit reversible networks (RevNets) to learn nonlinear level sets of a high-dimensional function and parameterize its level sets in low-dimensional spaces. A new loss function was designed to utilize samples of the target functions' gradient to encourage the transformed function to be sensitive to only a few transformed coordinates. The NLL approach is demonstrated by applying it to three 2D functions and two 20D functions for showing the improved approximation accuracy with the use of nonlinear transformation, as well as to an 8D composite material design problem for optimizing the buckling-resistance performance of composite shells of rocket inter-stages.",1902.10652v3 2015-06-29,Bilayer Insulator Tunnel Barriers for Graphene-Based Vertical Hot-electron Transistors,"Vertical graphene-based device concepts that rely on quantum mechanical tunneling are intensely being discussed in literature for applications in electronics and optoelectronics. In this work, the carrier transport mechanisms in semiconductor-insulator-graphene (SIG) capacitors are investigated with respect to their suitability as the electron emitter in vertical graphene base transistors (GBTs). Several dielectric materials as tunnel barriers are compared, including dielectric double layers. Using bilayer dielectrics, we experimentally demonstrate significant improvements in the electron injection current by promoting Fowler-Nordheim tunneling (FNT) and step tunneling (ST) while suppressing defect mediated carrier transports. High injected tunneling current densities approaching 10$^3$ A/cm$^2$ (limited by series resistance), and excellent current-voltage nonlinearity and asymmetry are achieved using a 1 nm-thick high quality dielectric, thulium silicate (TmSiO), as the first insulator layer, and titanium dioxide (TiO$_2$) as a high electron affinity second layer insulator. We also confirm the feasibility and effectiveness of our approach in a full GBT structure which shows dramatic improvement in the collector on-state current density with respect to the previously reported GBTs. The device design and the fabrication scheme have been selected with future CMOS process compatibility in mind. This work proposes a bilayer tunnel barrier approach as a promising candidate to be used in high performance vertical graphene-based tunneling devices.",1506.08721v2 2019-01-05,"Transmission lines and resonators based on quantum Hall plasmonics: electromagnetic field, attenuation and coupling to qubits","Quantum Hall edge states have some characteristic features that can prove useful to measure and control solid state qubits. For example, their high voltage to current ratio and their dissipationless nature can be exploited to manufacture low-loss microwave transmission lines and resonators with a characteristic impedance of the order of the quantum of resistance $h/e^2\sim 25\mathrm{k\Omega}$. The high value of the impedance guarantees that the voltage per photon is high and for this reason high impedance resonators can be exploited to obtain larger values of coupling to systems with a small charge dipole, e.g. spin qubits. In this paper, we provide a microscopic analysis of the physics of quantum Hall effect devices capacitively coupled to external electrodes. The electrical current in these devices is carried by edge magnetoplasmonic excitations and by using a semiclassical model, valid for a wide range of quantum Hall materials, we discuss the spatial profile of the electromagnetic field in a variety of situations of interest. Also, we perform a numerical analysis to estimate the lifetime of these excitations and, from the numerics, we extrapolate a simple fitting formula which quantifies the $Q$ factor in quantum Hall resonators. We then explore the possibility of reaching the strong photon-qubit coupling regime, where the strength of the interaction is higher than the losses in the system. We compute the Coulomb coupling strength between the edge magnetoplasmons and singlet-triplet qubits, and we obtain values of the coupling parameter of the order $100\mathrm{MHz}$; comparing these values to the estimated attenuation in the resonator, we find that for realistic qubit designs the coupling can indeed be strong.",1901.01455v1 2020-01-16,Anisotropic character of the metal-to-metal transition in Pr4Ni$_3$O$_{10}$,"As a member of the Ruddlesden-Popper Ln$_{n+1}$Ni$_n$O$_{3n+1}$ series rare-earth-nickelates, the Pr4Ni$_3$O$_{10}$ consists of infinite quasi-two-dimensional perovskite-like Ni-O based layers. Although a metal-to-metal phase transition at Tpt = 157 K has been revealed by previous studies, a comprehensive study of physical properties associated with this transition has not yet been performed. We have grown single crystals of Pr4Ni3O10 at high oxygen pressure, and report on the physical properties around that phase transition, such as heat-capacity, electric-transport and magnetization. We observe a distinctly anisotropic behavior between in-plane and out-of-plane properties: a metal-to-metal transition at Tpt within the a-b plane, and a metal-to-insulator-like transition along the c-axis with decreasing temperature. Moreover, an anisotropic and anomalous negative magneto-resistance is observed at Tpt that we attribute to a slight suppression of the first-order transition with magnetic field. The magnetic-susceptibility can be well described by a Curie-Weiss law, with different Curie-constants and Pauli-spin susceptibilities between the high-temperature and the low-temperature phases. The single crystal X-ray diffraction measurements show a shape variation of the different NiO6 octahedra from the high-temperature phase to the low-temperature phase. This subtle change of the environment of the Ni sites is likely responsible for the different physical properties at high and low temperatures.",2001.05916v2 2020-06-08,200 mm Sensor Development Using Bonded Wafers,"Sensors fabricated from high resistivity, float zone, silicon material have been the basis of vertex detectors and trackers for the last 30 years. The areas of these devices have increased from a few square cm to $\> 200\ m^2$ for the existing CMS tracker. High Luminosity Large Hadron Collider (HL-LHC), CMS and ATLAS tracker upgrades will each require more than $200\ m^2$ of silicon and the CMS High Granularity Calorimeter (HGCAL) will require more than $600\ m^2$. The cost and complexity of assembly of these devices is related to the area of each module, which in turn is set by the size of the silicon sensors. In addition to large area, the devices must be radiation hard, which requires the use of sensors thinned to 200 microns or less. The combination of wafer thinning and large wafer diameter is a significant technical challenge, and is the subject of this work. We describe work on development of thin sensors on $200 mm$ wafers using wafer bonding technology. Results of development runs with float zone, Silicon-on-Insulator and Silicon-Silicon bonded wafer technologies are reported.",2006.04888v2 2021-02-11,High-Mobility p-Channel Wide Bandgap Transistors Based on h-BN/Diamond Heterostructures,"Field-effect transistors made of wide-bandgap semiconductors can operate at high voltages, temperatures and frequencies with low energy losses, and have been of increasing importance in power and high-frequency electronics. However, the poor performance of p-channel transistors compared with that of n-channel transistors has constrained the production of energy-efficient complimentary circuits with integrated n- and p-channel transistors. The p-type surface conductivity of hydrogen-terminated diamond offers great potential for solving this problem, but surface transfer doping, which is commonly believed to be essential for generating the conductivity, limits the performance of transistors made of hydrogen-terminated diamond because it requires the presence of ionized surface acceptors, which cause hole scattering. Here, we report on fabrication of a p-channel wide-bandgap heterojunction field-effect transistor consisting of a hydrogen-terminated diamond channel and hexagonal boron nitride ($h$-BN) gate insulator, without relying on surface transfer doping. Despite its reduced density of surface acceptors, the transistor has the lowest sheet resistance ($1.4$ k$\Omega$) and largest on-current ($1600$ $\mu$m mA mm$^{-1}$) among p-channel wide-bandgap transistors, owing to the highest hole mobility (room-temperature Hall mobility: $680$ cm$^2$V$^{-1}$s$^{-1}$). Importantly, the transistor also shows normally-off behavior, with a high on/off ratio exceeding $10^8$. These characteristics are suited for low-loss switching and can be explained on the basis of standard transport and transistor models. This new approach to making diamond transistors paves the way to future wide-bandgap semiconductor electronics.",2102.05982v2 2021-03-30,High-Tc superconductivity in clathrate calcium hydride CaH6,"Recent discovery of superconductive rare earth/actinide superhydrides has ushered in a new era of superconductivity research at high pressures. This distinct type of clathrate metal hydrides was first proposed for alkaline-earth-metal hydride CaH6 that, however, has long eluded experimental synthesis, impeding an understanding of pertinent physics. Here, we report successful synthesis of CaH6 and its measured superconducting critical temperature Tc of 215 K at 172 GPa, which is evidenced by a sharp drop of resistivity to zero and a characteristic decrease of Tc under a magnetic field up to 9 T.An estimate based on the Werthamer-Helfand-Hohenberg model gives a giant zero-temperature upper critical magnetic field of 203 T. These remarkable benchmark superconducting properties place CaH6 among the most outstanding high-Tc superhydrides, marking it as the hitherto only clathrate metal hydride outside the family of rare earth/actinide hydrides. This exceptional case raises great prospects of expanding the extraordinary class of high-Tc superhydrides to a broader variety of compounds that possess more diverse material features and physics characteristics.",2103.16282v3 2022-12-28,Superconductivity Observed in Tantalum Polyhydride at High Pressure,"We report experimental discovery of tantalum polyhydride superconductor. It was synthesized at high pressure and high temperature conditions using diamond anvil cell combined with in-situ high pressure laser heating techniques. The superconductivity was investigated via resistance measurements at pressures. The highest superconducting transition temperature Tc was found to be ~30 K at 197 GPa in the sample that was synthesized at the same pressure with ~2000 K heating. The transitions are shifted to low temperature upon applying magnetic fields that supports the superconductivity nature. The upper critical field at zero temperature {\mu}0Hc2(0) of the superconducting phase is estimated to be ~20 T that corresponds to GL coherent length ~40 angstroms. Our results suggest that the superconductivity may arise from I-43d phase of TaH3. It is, for the first time to our best knowledge, experimental realization of superconducting hydrides for the VB group of transitional metals.",2212.13739v3 2024-02-19,Cross talk of a large-scale depleted monolithic active pixel sensor (DMAPS) in 180 nm CMOS technology,"Monolithic pixel detectors combine readout electronics and sensor in a single entity of silicon, which simplifies the production procedure and lowers the material budget compared to conventional hybrid pixel detector concepts. Benefiting from the advances in commercial CMOS processes towards large biasing voltage capabilities and the increasing availability of high-resistivity substrates, depleted monolithic active pixel sensors (DMAPS) are able to cope with the high-rate and high-radiation environments faced in modern high-energy physics experiments. TJ-Monopix2 is the latest iteration of a DMAPS development line designed in 180 nm TowerSemicondutor technology, which features a large scale (2 x 2) cm$^2$ chip divided into (512 x 512) pixels with a pitch of (33 x 33) um$^2$. All in-pixel electronics are separated from its small collection electrode and process modifications are implemented to improve charge collection efficiency especially after irradiation. The latest laboratory measurements and investigations of a threshold variation observed for TJ-Monopix2 in typical operating conditions are presented.",2402.12153v1 2019-02-08,Investigating Short-term and Long-term Binder Performance of High-RAP Mixtures Containing Waste Cooking Oil,"The environmental and economic benefits of recycling asphalt pavements have received much attention in recent years. Because of the increase in the cost of raw materials and energy carriers, the reuse of large portions of reclaimed asphalt pavement (RAP) is critical in reducing both the cost and environmental footprint of asphalt pavements. High-RAP mixtures are more prone to low temperature cracking and poor mixture workability because of the higher stiffness of RAP binder. Recycling agents are one of the additives which are used to improve these deficiencies. However, there is some ambiguity about the optimum content of recycling agent to assure proper performance of recycled asphalt pavement during its service life. The current study used 60% and 100% fractionated RAP with waste cooking oil as a recycling agent and crumb rubber to alleviate the aforementioned problems. Laboratory evaluation showed that increasing the amount of recycling agent in the high-RAP mixtures improved their workability and low temperature performance while decreasing moisture damage and rutting resistance. The long-term susceptibility to aging of recycled binder with the organically-based recycling agent was also investigated. A procedure to obtain the optimum percentage of recycling agent was devised to strike a balance between the performance characteristics of mixtures with a high-RAP content.",1905.13701v1 2016-03-12,Complex structures of dense lithium: electronic origin,"Lithium - the lightest alkali metal - exhibits unexpected structures and electronic behaviour at high pressures. As the heavier alkalis, Li is bcc at ambient pressure and transforms first to fcc (at 7.5 GPa). The post-fcc high-pressure form Li-cI16 (at 40-60 GPa) is similar to Na-cI16 and related to more complex structures of heavy alkalis Rb-oC52 and Cs-oC84. The other high pressure phases for Li (oC88, oC40, oC24) found at pressures up to 130 GPa are specific the only to Li. The different route of Li high-pressure structures correlates with its special electronic configuration containing the only 3 electrons (at 1s and 2s levels). Crystal structures for Li are analyzed within the model of Fermi sphere - Brillouin zone interactions. Stability of post-fcc structures for Li can be supported by Hume-Rothery arguments when new Brillouin zone plains appear close to the Fermi level producing pseudogaps near the Fermi level and decreasing the crystal energy. The filling of Brillouin-Jones zones by electron states for a given structure defines the physical properties as optical reflectivity, electrical resistivity and superconductivity. To understand complexity of structural and physical properties of Li above 60 GPa is necessary to assume the valence electrons band overlap with the upper core electrons and increase the valence electron count under compression.",1603.03926v1 2019-03-28,High spin-polarization in the low Curie temperature complex itinerant ferromagnet EuTi$_{1-x}$Nb$_x$O$_3$,"The physical systems with ferromagnetism and ""bad"" metallicity hosting unusual transport properties are playgrounds of novel quantum phenomena. Recently EuTi$_{1-x}$Nb$_x$O$_3$ emerged as a ferromagnetic system where non-trivial temperature dependent transport properties are observed due to coexistence and competition of various magnetic and non-magnetic scattering processes. In the ferromagnetic state, the resistivity shows a $T^2$ temperature dependence possibly due to electron-magnon scattering and above the Curie temperature $T_c$, the dependence changes to $T^{3/2}$ behaviour indicating a correlation between transport and magnetic properties. In this paper, we show that the transport spin-polarization in EuTi$_{1-x}$Nb$_x$O$_3$, a low Curie temperature ferromagnet, is as high ($\sim 40\%$) as that in some of the metallic ferromagnets with high Curie temperatures. In addition, owing to the low Curie temperature of EuTi$_{1-x}$Nb$_x$O$_3$, the temperature ($T$) dependence of $P_t$ could be measured systematically up to $T_c$ which revealed a proportionate relationship with magnetization $M_s$ vs. $T$. This indicates that such proportionality is far more universally valid than the ferromagnets with ideal parabolic bands. Furthermore, our band structure calculations not only helped understand the origin of such high spin polarization in EuTi$_{1-x}$Nb$_x$O$_3$ but also provided a route to estimate the Hubbard $U$ parameter in complex metallic ferromagnets in general using experimental inputs.",1903.12022v1 2011-04-22,Can nothing be a superconductor and a superfluid?,"A superconductor is a material that conducts electric current with no resistance. Superconductivity and magnetism are known to be antagonistic phenomena: superconductors expel weak external magnetic field (the Meissner effect) while a sufficiently strong magnetic field, in general, destroys superconductivity. In a seemingly contradictory statement, we show that a very strong magnetic field can turn an empty space into a superconductor. The external magnetic field required for this effect should be about 10^{16} Tesla (eB ~ 1 GeV^2). The physical mechanism of the exotic vacuum superconductivity is as follows: in strong magnetic field the dynamics of virtual quarks and antiquarks is effectively one-dimensional because these electrically charged particles tend to move along the lines of the magnetic field. In one spatial dimension a gluon-mediated attraction between a quark and an antiquark of different flavors inevitably leads to formation of a colorless spin-triplet bound state (a vector analogue of the Cooper pair) with quantum numbers of an electrically charged rho meson. Such quark-antiquark pairs condense to form an anisotropic inhomogeneous superconducting state similar to the Abrikosov vortex lattice in a type-II superconductor. The onset of the superconductivity of the charged rho mesons should also induce an inhomogeneous superfluidity of the neutral rho mesons. The vacuum superconductivity should survive at very high temperatures of typical Quantum Chromodynamics (QCD) scale of 10^{12} K (T ~ 100 MeV). We propose the phase diagram of QCD in the plane ""magnetic field - temperature"".",1104.4404v1 2019-06-14,Tunneling Magnetoresistance and Spin-Dependent Diode Performance in Fully Epitaxial Magnetic Tunnel Junctions with Rock-salt Type ZnO/MgO,"We fabricate fully epitaxial Fe/ZnO/MgO/Fe magnetic tunnel junctions (MTJs) with a bilayer tunnel barrier, in which ZnO has a metastable rock-salt crystal structure. We observe a high magnetoresistance ratio up to 96% at room temperature (RT) and find that these MTJs have asymmetric current-voltage characteristics, and their rectifying performances are largely dependent on the magnetization alignments of the Fe electrodes. Diode responsibilities at a zero-bias voltage ($\beta_{0}$), which is an important performance index for harvesting applications, are observed up to 1.3 A/W at RT in the antiparallel alignment of the magnetizations while maintaining rather low resistance-area (RA) products (a few tens of k${\Omega\mu}$m$^2$). Even with the same top and bottom electrodes (Fe), the obtained $\beta_{0}$ values are comparable to those of reported high-performance tunnel diodes consisting of amorphous bilayer tunnel barriers with polycrystalline dissimilar electrodes. This strongly suggests that the epitaxial ZnO/MgO bilayer tunnel barrier is effective for enhancing the $\beta_{0}$ without significant increase in the RA. In addition, we demonstrate that a zero-bias anomaly in thetunnel conductance, which originates from the magnon excitations at the Fe/barrier interfaces, plays a crucial role in observed spin-dependent diode performance. The results indicate that a fully epitaxial MTJ with a bilayer tunnel barrier is a promising candidate to establish a high-performance high-frequency rectifying system.",1906.05981v1 2020-11-24,Inkjet printed circuits with two-dimensional semiconductor inks for high-performance electronics,"Air-stable semiconducting inks suitable for complementary logic are key to create low-power printed integrated circuits (ICs). High-performance printable electronic inks with two-dimensional materials have the potential to enable the next generation of high performance, low-cost printed digital electronics. Here we demonstrate air-stable, low voltage (< 5 V) operation of inkjet-printed n-type molybdenum disulfide (MoS2) and p-type indacenodithiophene-co-benzothiadiazole (IDT-BT) field-effect transistors (FETs), estimating a switching time of {\tau} ~ 3.3 {\mu}s for the MoS2 FETs. We achieve this by engineering high-quality MoS2 and air-stable IDT-BT inks suitable for inkjet-printing complementary pairs of n-type MoS2 and p-type IDT-BT FETs. We then integrate MoS2 and IDT-BT FETs to realise inkjet-printed complementary logic inverters with a voltage gain |Av| ~ 4 when in resistive load configuration and |Av| ~ 1.36 in complementary configuration. These results represent a key enabling step towards ubiquitous long-term stable, low-cost printed digital ICs.",2011.12359v1 2020-11-26,A two-dimensional electron gas based on a 5s oxide with high room-temperature mobility and strain sensitivity,"The coupling of optical and electronic degrees of freedom together with quantum confinement in low-dimensional electron systems is particularly interesting for achieving exotic functionalities in strongly correlated oxide electronics. Recently, high room-temperature mobility has been achieved for a large bandgap transparent oxide - BaSnO$_3$ upon extrinsic La or Sb doping, which has excited significant research attention. In this work, we report the observation of room-temperature ferromagnetism in BaSnO$_3$ thin films and the realization of a two-dimensional electron gas (2DEG) on the surface of transparent BaSnO$_3$ via oxygen vacancy creation, which exhibits a high carrier density of $\sim 7.72*10^{14} /{\rm cm}^2$ and a high room-temperature mobility of ~18 cm$^2$/V/s. Such a 2DEG is rather sensitive to strain and a less than 0.1% in-plane biaxial compressive strain leads to a giant resistance enhancement of 350% (more than 540 kOhm/Square) at room temperature. Thus, this work creates a new path to exploring the physics of low-dimensional oxide electronics and devices applicable at room temperature.",2011.13106v2 2021-06-17,Quasi-solid-state sodium-ion hybrid capacitors enabled by UiO-66@PVDF-HFP multifunctional separators: selective charge transfer and high safety,"The practical application of sodium-ion hybrid capacitors is limited by their low energy densities resulted from the kinetics mismatch between cathodes and anodes, and the fire safety related to the flammable electrolyte-separator system. Hence, we report a rational design of metal-organic frameworks (MOFs, UiO-66) modified PVDF-HFP separator. High tensile strength and dimensional thermal stability of the separator reduce the risk of electrode short circuit caused by the separator deformation. MCC test demonstrates a reduction of 75% in peak heat release rate (pHRR), indicating an enhanced fire-resistant property of the separator. This is due to the transformation of UiO-66 into ZrO2 accompanied by the consumption of oxygen and the formation of the barrier char that suppresses further heat release. Quasi-solid-state electrolyte prepared based on this separator presents an enhanced ionic conductivity of 2.44 mS*cm-1 and Na-ion transference number of 0.55, which are related to the high porosity ( >70%) and electrolyte uptake (~ 320%) of the separator. Moreover, the open metal sites of UiO-66 can capture PF6- and consequently liberate the Na+ for faster migration, thus reducing the kinetics mismatch between cathodes and anodes. Such multifunctional separator enables the quasi-solid-state Na-ion hybrid capacitor to achieve high energy density (182 Wh*kg-1 @31 W*kg-1) and power density (5280 W*kg-1 @22 Wh*kg-1), as well as excellent cyclic stability (10000 cycles @1000 mA*g-1). Keywords: Quasi-solid-state; PVDF-HFP; Metal-organic frameworks; Dimensional thermal stability; Fire safety; Selective charge transfer",2106.09654v1 2021-12-13,Robustness of superconductivity to external pressure in high-entropy-alloy-type metal telluride AgInSnPbBiTe5,"High-entropy-alloy (HEA) superconductors are a new class of disordered superconductors. In this study, we investigate the robustness of superconducting states in HEA-type metal telluride (MTe; M = Ag, In, Sn, Pb, Bi) under high pressure. PbTe exhibits a structural transition from a NaCl-type to an orthorhombic Pnma structure at low pressures, and further transitions to a CsCl-type structure at high pressures. When the superconductivity of the CsCl-type PbTe is observed, it is found that its superconducting transition temperature (Tc) decreases with pressure. However, in the HEA-type AgInSnPbBiTe5, Tc is almost independent of pressure, for pressures ranging from 13.0 to 35.1 GPa. This trend is quite similar to that observed in an HEA superconductor (TaNb)0.67(HfZrTi)0.33, which shows that the robustness of superconductivity to external pressure is a universal feature in HEA-type superconductors. To clarify the effects of the modification of the configurational entropy of mixing on the crystal structure, superconducting states, and electronic structure of MTe, electrical resistance measurements, synchrotron X-ray diffraction, and synchrotron X-ray absorption spectroscopy with partial fluorescence mode (PFY-XAS) for three MTe polycrystalline samples of PbTe, AgPbBiTe3, and AgInSnPbBiTe5 with different configurational entropies of mixing at the M site were performed.",2112.06461v1 2022-12-12,Robust superconductivity and fragile magnetism induced by the strong Cu impurity scattering in the high-pressure phase of FeSe,"Superconductivity in FeSe is strongly enhanced under applied pressure and it is proposed to emerge from anomalously coupled structural and magnetic phases. Small impurities inside the Fe plane can strongly disrupt the pair formation in FeSe at ambient pressure and can also reveal the interplay between normal and superconducting phases. Here, we investigate how an impurity inside the Fe plane induced by the Cu substitution can alter the balance between competing electronic phases of FeSe at high pressures. In the absence of an applied magnetic field, at low pressures the nematic and superconducting phases are suppressed by a similar factor. On the other hand, at high pressures, above 10 kbar, the superconductivity remains unaltered despite the lack of any signature in transport associated to a magnetic phase in zero-magnetic field. However, by applying a magnetic field, the resistivity displays an anomaly preceding the activated behaviour in temperature, assigned to a magnetic anomaly. We find that the high-pressure superconducting phase of FeSe is robust and remains enhanced in the presence of Cu impurity, whereas the magnetic phase is not. This could suggest that high-$T_{\rm c}$ superconductivity has a sign-preserving order parameter in a presence of a rather glassy magnetic phase.",2212.06128v1 2023-01-30,Semimetal-Monolayer Transition Metal Dichalcogenides Photodetectors for Wafer-Scale Ultraviolet Photonics,"Atomically thin two-dimensional (2D) transition metal dichalcogenides (TMDs), such as MoS$_2$, are promising candidates for nanoscale photonics because of strong-light matter interactions. However, Fermi level pinning due to metal-induced gap (MIGS) states at the metals-monolayer MoS$_2$ interface limits the application of optoelectronic devices based on conventional metals because of the high contact resistance of the Schottky contacts. On the other hand, a semimetal-TMD-semimetal device can overcome this limitation, where the MIGS are sufficiently suppressed and can result in ohmic contacts. Here we demonstrate the optoelectronic performance of a bismuth-monolayer (1L) MoS$_2$-bismuth device with ohmic electrical contacts and extraordinary optoelectronic properties. To address the wafer-scale production, we grew full coverage 1L MoS$_2$ by using chemical vapor deposition method. We measured high photoresponsivity of 300 A/W in the UV regime at 77 K, which translates into an external quantum efficiency (EQE) ~ 1000 or $10^5$%. We found that the 90% rise time of our devices at 77 K is 0.1 ms, which suggests that the current devices can operate at the speed of ~ 10 kHz. The combination of large-array device fabrication, high sensitivity, and high-speed response offers great potential for applications in photonics that includes integrated optoelectronic circuits.",2301.12635v1 2023-04-13,Self-doping effect in confined copper selenide semiconducting quantum dots for efficient photoelectrocatalytic oxygen evolution,"Self-doping can not only suppress the photogenerated charge recombination of semiconducting quantum dots by self-introducing trapping states within the bandgap, but also provide high-density catalytic active sites as the consequence of abundant non-saturated bonds associated with the defects. Here, we successfully prepared semiconducting copper selenide (CuSe) confined quantum dots with abundant vacancies and systematically investigated their photoelectrochemical characteristics. Photoluminescence characterizations reveal that the presence of vacancies reduces the emission intensity dramatically, indicating a low recombination rate of photogenerated charge carriers due to the self-introduced trapping states within the bandgap. In addition, the ultra-low charge transfer resistance measured by electrochemical impedance spectroscopy implies the efficient charge transfer of CuSe semiconducting quantum dots-based photoelectrocatalysts, which is guaranteed by the high conductivity of their confined structure as revealed by room-temperature electrical transport measurements. Such high conductivity and low photogenerated charge carriers recombination rate, combined with high-density active sites and confined structure, guaranteeing the remarkable photoelectrocatalytic performance and stability as manifested by photoelectrocatalysis characterizations. This work promotes the development of semiconducting quantum dots-based photoelectrocatalysis and demonstrates CuSe semiconducting quantum confined catalysts as an advanced photoelectrocatalysts for oxygen evolution reaction.",2304.06422v1 2009-12-15,Kondo effect and absence of quantum interference effects in the charge transport of cobalt doped iron pyrite,"The Hall effect and resistivity of the carrier doped magnetic semiconductor Fe$_{1-x}$Co$_x$S$_2$ were measured for $0\le x \le 0.16$, temperatures between 0.05 and 300 K, and fields of up to 9 T. Our Hall data indicate electron charge carriers with a density of only 10 to 30% of the Co density of our crystals. Despite the previous identification of magnetic Griffiths phase formation in the magnetic and thermodynamic properties of this system for the same range of $x$, we measure a temperature independent resistivity below 0.5 K indicating Fermi liquid-like transport. We also observe no indication of quantum corrections to the conductivity despite the small values of the product of the Fermi wave vector and the mean-free-path, $1.5 \le k_F\ell \le 15$, over the range of $x$ investigated. This implies a large inelastic scattering rate such that the necessary condition for the observation of quantum contributions to the carrier transport, quantum coherence over times much longer than the elastic scattering time, is not met in our samples. Above 0.5 K we observe a temperature and magnetic field dependent resistivity that closely resembles a Kondo anomaly for $x$ less than that required to form a long range magnetic state, $x_c$. For $x>x_c$, the resistivity and magnetoresistance resemble that of a spin glass with a reduction of the resistivity by as much as 35% in 5 T fields. We also observe an enhancement of the residual resistivity ratio by almost a factor of 2 for samples with $x\sim x_c$ indicating temperature dependent scattering mechanisms beyond simple carrier-phonon scattering. We speculate that this enhancement is due to charge carrier scattering from magnetic fluctuations which contribute to the resistivity over a wide temperature range.",0912.2980v1 2022-01-04,Superior effect of edge relative to basal plane functionalization of graphene in enhancing polymer-graphene nanocomposite thermal conductivity-A combined molecular dynamics and Greens functions study,"To achieve high thermal conductivity (k) of polymer graphene nanocomposites, it is critically important to achieve efficient thermal coupling between graphene and its surrounding polymers through effective functionalization schemes. In this work, we demonstrate that edge-functionalization of graphene nanoplatelets (GnPs) can enable a larger enhancement of effective thermal conductivity in polymer-graphene nanocomposites, relative to basal plane functionalization. Effective thermal conductivity for edge case is predicted, through molecular dynamics simulations, to be up to 48% higher relative to basal plane bonding for 35 wt.% graphene loading with 10 layers thick nanoplatelets. This unique result opens up promising new avenues for achieving high thermal-conductivity polymer materials, which is of key importance for a wide range of thermal management technologies. The anisotropy of thermal transport in single layer graphene leads to very high in-plane thermal conductivity (~2000 W/mK) compared to the low out-of-plane thermal conductivity (~10 W/mK). Likewise, in multilayer graphene nanoplatelet (GnP), the thermal conductivity across the layers is even lower due to the weak van der Waals bonding between each pair of layers. Edge functionalization couples the polymer chains to the high in-plane thermal conduction pathway of graphene, thus leading to high overall high composite thermal conductivity. Basal-plane functionalization, however, lowers the thermal resistance between the polymer and the surface graphene sheets of the nanoplatelet only, causing the heat conduction through inner layers to be less efficient, thus resulting in basal plane scheme to be outperformed by edge scheme. The present study fundamentally enables novel pathways for achieving high thermal-conductivity polymer composites.",2201.01011v1 2008-11-14,Electronic transport in ferromagnetic alloys and the Slater-Pauling Curve,"Experimental measurements of the residual resistivity $\rho(x)$ of the binary alloy system Fe$_{1-x}$Cr$_x$ have shown an anomalous concentration dependence which deviates significantly from Nordheim's rule. In the low ($x < 10%$) Cr concentration regime the resistivity has been found to increase linearly with $x$ until $\approx$ 10% Cr where the resistivity reaches a plateau persisting to $\approx$ 20% Cr. In this paper we present $ab$-$initio$ calculations of $\rho(x)$ which explain this anomalous behavior and which are based on the Korringa-Kohn-Rostoker (KKR) method in conjunction with the Kubo-Greenwood formalism. Furthermore we are able to show that the effects of short-range ordering or clustering have little effect via our use of the nonlocal coherent-potential approximation (NL-CPA). For the interpretation of the results we study the alloys' electronic structure by calculating the Bloch spectral function particularly in the vicinity of the Fermi energy. From the analysis of our results we infer that a similar behavior of the resistivity should also be obtained for iron-rich Fe$_{1-x}$V$_x$ alloys - an inference confirmed by further explicit resistivity calculations. Both of these alloy systems belong to the same branch of the famous Slater-Pauling plot and we postulate that other alloy systems from this branch should show a similar behavior. Our calculations show that the appearance of the plateau in the resistivity can be attributed to the dominant contribution of minority spin electrons to the conductivity which is nearly unaffected by increase in Cr/V concentration $x$ and we remark that this minority spin electron feature is also responsible for the simple linear variation of the average moment in the Slater-Pauling plot for these materials.",0811.2303v1 2020-12-11,Improving fretting corrosion resistance of CoCrMo alloy with TiSiN and ZrN coatings for orthopedic applications,"Total hip replacement is the most effective treatment for late stage osteoarthritis. However, adverse local tissue reactions (ALTRs) associated with fretting corrosion have been observed in patients with modular total hip implants. The purpose of this study is to increase the fretting corrosion resistance of the CoCrMo alloy and the associated metal ion release by applying hard coatings to the surface. Cathodic arc evaporation technique (arc-PVD) was used to deposit TiSiN and ZrN hard coatings on to CoCrMo substrates. The morphology, chemical composition, crystal structures and residual stress of the coatings were characterized by scanning electron microscopy, energy dispersive x-ray spectroscopy, and X-ray diffractometry. Hardness, elastic modulus, and adhesion of the coatings were measured by nano-indentation, nano-scratch test, and the Rockwell C test. Fretting corrosion resistance tests of coated and uncoated CoCrMo discs against Ti6Al4V spheres were conducted on a four-station fretting testing machine in simulated body fluid at 1Hz for 1 million cycles. Post-fretting samples were analyzed for morphological changes, volume loss and metal ion release. Our analyses showed better surface finish and lower residual stress for ZrN coating, but higher hardness and better scratch resistance for TiSiN coating. Fretting results demonstrated substantial improvement in fretting corrosion resistance of CoCrMo with both coatings. ZrN and TiSiN decreased fretting volume loss by more than 10 times and 1000 times, respectively. Both coatings showed close to 90% decrease of Co ion release during fretting corrosion tests. Our results suggest that hard coating deposition on CoCrMo alloy can significantly improve its fretting corrosion resistance and could thus potentially alleviate ALTRs in metal hip implants.",2012.06614v1 2018-03-06,Approach combining the Rietveld method and pairs distribution function analysis to study crystalline materials under high-pressure and/or temperature: Application to rhombohedral Bi2Te3 phase,"An approach combining the Rietveld method and pairs distribution function analysis to study crystalline materials under high pressure or temperature was early proposed by us, and in this study, it was applied to investigate de effect of high pressure on the rhombohedral Bi2Te3 phase. The refined structural parameters obtained from the Rietveld refinement of the XRD patterns measured for pressures up to 9.1 GPa were used as input data to simulate the partial and total structure factors SBiBi, SBiTe, STeTe, and SBi2Te3. Fourier transformation of the Sij factors permitted to obtain the partial and total pairs distribution functions GBiBi, GBiTe, GTeTe, and GBi2Te3. The first coordination shells of these Gij functions are formed by subshells and, with increasing pressure in the 1.1 to 6.3 GPa range, occur a partial separation of subshells. Also, the increase of pressure in this range promotes a drastic reduction in the values of the intralayer angles TeBiTe, and consequently, in the intralayer distance TeTe. A drastic reduction in the interlayers distance Te-Te was also observed. Several studies are reported in the literature, including one carried out by us, show the presence of an ETT in this pressure range. The obtained results suggest that the ETT is related with the decrease of the intralayer angles TeBiTe, and intra- and interlayer distance TeTe. Experimental results describing the pressure dependence the thermoelectric power, electrical resistivity, and power fator for rhombohedral Bi2Te3 are reported, and an enhancement of the power factor in the 1.1 to 6.3 GPa range is observed. The results obtained in this study give evidence that this enhancement in the power factor is related with the decrease of the intralayer angles TeBiTe, and with the decrease of intralayer- and interlayers homopolar TeTe bonds.",1803.02479v1 2021-01-30,Fast drying of high-alumina MgO-bonded refractory castables,"Refractory producers face many challenges in terms of producing MgO-containing castables due to the high likelihood of magnesia to hydrate in contact with water, resulting in Mg(OH)2 generation. The expansive feature of this transformation affects the performance of such refractories, as (i) if this hydrated phase is not accommodated in the formed microstructure, ceramic linings with cracks and low green mechanical strength will be obtained; and (ii) if crack-free pieces are prepared, they should present low porosity and reduced permeability, which require special attention when heating these materials. This work investigated the ability of various additives in the optimization of the drying behavior of Al2O3-MgO castables. Vibratable compositions were tested after incorporating polymeric fibers (PF), an organic salt (OAS), SiO2-based additive (SM) or permeability enhancing active compound (MP) into the dry-mixtures. Various experimental measurements were performed to infer the role of the drying agents to prevent the samples explosion and whether they would also influence other properties of the castables. As observed, OAS and MP helped to inhibit the MgO-bonded samples explosion even under severe heating conditions (2-20C/min) and increased their green mechanical strength and slag infiltration resistance when compared to the additive-free composition. On the other hand, the addition of polymeric fibers (PF) or silica-based compound (SM) to the formulations was not able to prevent the castables explosion when using a high heating rate and other side effects could also be observed when testing these materials. Thus, the selection of suitable drying agents is a key issue, as they may allow the development of MgO-bonded castables with enhanced properties and lower spalling risk during their first thermal treatment.",2102.00217v1 2022-03-14,Revisiting stress-corrosion cracking and hydrogen embrittlement in 7xxx-Al alloys at the near-atomic-scale,"Hydrogen embrittlement (HE) affects all major high-strength structural materials and as such is a major impediment to lightweighting e.g. vehicles and help reduce carbon-emissions and reach net-zero. The high-strength 7xxx series aluminium alloys can fulfil the need for light, high strength materials, and are already extensively used in aerospace for weight reduction purposes. However, depending on the thermomechanical and loading state, these alloys can be sensitive to stress-corrosion cracking (SCC) through anodic dissolution and hydrogen embrittlement. Here, we study at the near-atomic-scale the intra- and inter-granular microstructure ahead and in the wake of a propagating SCC crack. Moving away from model cases not strictly relevant to application, we performed an industry-standard test on an engineering Al-7XXX alloy. H is found segregated to planar arrays of dislocations and to grain boundaries that we can associate to the combined effects of hydrogen-enhanced localized plasticity (HELP) and hydrogen-enhanced decohesion (HEDE) mechanisms. We report on a Mg-rich H-rich amorphous oxide on the corroded crack surface and evidence of Mg-related diffusional processes leading to dissolution of the strengthening eta-phase precipitates ahead of the crack. We show ingress of up to 1 at% O, i.e. well above the solubility limit of O in Al, near the oxide-metal interface, while no increased level of H is found in the matrix. We provide an array of discussion points relative to the interplay of structural defects, transport of solutes, thereby changing the resistance against crack propagation, which have been overlooked across the SCC literature and prevent accurate service life predictions.",2203.07058v1 2022-04-06,First principles investigation of anionic redox in bisulfate lithium battery cathodes,"The search for an alternative high-voltage polyanionic cathode material for Li-ion batteries is vital to improve the energy densities beyond the state-of-the-art, where sulfate frameworks form an important class of high-voltage cathode materials due to the strong inductive effect of the S$^{6+}$ ion. Here, we have investigated the mechanism of cationic and/or anionic redox in Li$_x$M(SO$_4$)$_2$ frameworks (M = Mn, Fe, Co, and Ni and 0 $\leq$ x $\leq$ 2) using density functional calculations. Specifically, we have used a combination of Hubbard $U$ corrected strongly constrained and appropriately normed (SCAN+$U$) and generalized gradient approximation (GGA+$U$) functionals to explore the thermodynamic (polymorph stability), electrochemical (intercalation voltage), geometric (bond lengths), and electronic (band gaps, magnetic moments, charge populations, etc.) properties of the bisulfate frameworks considered. Importantly, we find that the anionic (cationic) redox process is dominant throughout delithiation in the Ni (Mn) bisulfate, as verified using our calculated projected density of states, bond lengths, and on-site magnetic moments. On the other hand, in Fe and Co bisulfates, cationic redox dominates the initial delithiation (1 $\leq$ x $\leq$ 2), while anionic redox dominates subsequent delithiation (0 $\leq$ x $\leq$ 2). In addition, evaluation of the crystal overlap Hamilton population reveals insignificant bonding between oxidizing O atoms throughout the delithiation process in the Ni bisulfate, indicating robust battery performance that is resistant to irreversible oxygen evolution. Finally, we observe both GGA+$U$ and SCAN+$U$ predictions are in qualitative agreement for the various properties predicted. Our work should open new avenues for exploring lattice oxygen redox in novel high voltage polyanionic cathodes, especially using the SCAN+$U$ functional.",2204.02673v1 2012-09-07,Phase relations in K_xFe_{2-y}Se_2 and the structure of superconducting K_xFe_2Se_2 via high-resolution synchrotron diffraction,"Superconductivity in iron selenides has experienced a rapid growth, but not without major inconsistencies in the reported properties. For alkali-intercalated iron selenides, even the structure of the superconducting phase is a subject of debate, in part because the onset of superconductivity is affected much more delicately by stoichiometry and preparation than in cuprate or pnictide superconductors. If high-quality, pure, superconducting intercalated iron selenides are ever to be made, the intertwined physics and chemistry must be explained by systematic studies of how these materials form and by and identifying the many coexisting phases. To that end, we prepared pure K_2Fe_4Se_5 powder and superconductors in the K_xFe_{2-y}Se_2 system, and examined differences in their structures by high-resolution synchrotron and single-crystal x-ray diffraction. We found four distinct phases: semiconducting K_2Fe_4Se_5, a metallic superconducting phase K_xFe_2Se_2 with x ranging from 0.38 to 0.58, an insulator KFe_{1.6}Se_2 with no vacancy ordering, and an oxidized phase K_{0.51(5)}Fe_{0.70(2)}Se that forms the PbClF structure upon exposure to moisture. We find that the vacancy-ordered phase K_2Fe_4Se_5 does not become superconducting by doping, but the distinct iron-rich minority phase K_xFe_2Se_2 precipitates from single crystals upon cooling from above the vacancy ordering temperature. This coexistence of metallic and semiconducting phases explains a broad maximum in resistivity around 100 K. Further studies to understand the solubility of excess Fe in the K_xFe_{2-y}Se_2 structure will shed light on the maximum fraction of superconducting K_xFe_2Se_2 that can be obtained by solid state synthesis.",1209.1650v1 2015-04-10,Esaki diodes in van der Waals heterojunctions with broken-gap energy band alignment,"Van der Waals (vdW) heterojunctions composed of 2-dimensional (2D) layered materials are emerging as a solid-state materials family that exhibit novel physics phenomena that can power high performance electronic and photonic applications. Here, we present the first demonstration of an important building block in vdW solids: room temperature (RT) Esaki tunnel diodes. The Esaki diodes were realized in vdW heterostructures made of black phosphorus (BP) and tin diselenide (SnSe2), two layered semiconductors that possess a broken-gap energy band offset. The presence of a thin insulating barrier between BP and SnSe2 enabled the observation of a prominent negative differential resistance (NDR) region in the forward-bias current-voltage characteristics, with a peak to valley ratio of 1.8 at 300 K and 2.8 at 80 K. A weak temperature dependence of the NDR indicates electron tunneling being the dominant transport mechanism, and a theoretical model shows excellent agreement with the experimental results. Furthermore, the broken-gap band alignment is confirmed by the junction photoresponse and the phosphorus double planes in a single layer of BP are resolved in transmission electron microscopy (TEM) for the first time. Our results represent a significant advance in the fundamental understanding of vdW heterojunctions, and widen the potential applications base of 2D layered materials.",1504.02810v5 2018-12-01,Extrinsic n-type semiconductor transition in ZrSe2 with the metallic character through hafnium substitution,"Two dimensional layered materials exhibit versatile electronic properties in their different phases. The intrinsic electronic properties of these materials can be modulated through doping or intercalation. In this study, we investigated the electronic properties of Hf doped ZrSe2 single crystals using angle-resolved photoemission spectroscopy (ARPES) combined with first principles density functional theory (DFT) calculations. It is observed that the valence band maxima of ZrSe2, located below the Fermi level, undergo a significant change with the introduction of Hf substitution. Hf can introduce extra charges into the conduction band, rather than making a mixed structure of HfSe2 and ZrSe2 band structure, which can cross the Fermi level. Compared to the semiconducting band structure of ZrSe2, we observed that the conduction band crosses the Fermi level at the high symmetry M point in Hf-doped ZrSe2. This suggests an increase of electron type carriers around the Fermi level, resulting in an extrinsic charge carrier density in the conduction band, which can form a metallic behaviour. It can be noticed that the Hf cations can create disorder in the form of excess atoms of Zr, which yields more carriers in the conduction band in the shape of smeared bands. The tails of the smeared band occupied the d-orbitals extended into the Fermi level and left the d band below. Similarly, the electrical resistance measurements further confirm the metallic-like character of Hf doped ZrSe2 compared to the semiconductor ZrSe2, indicating increased carriers. This metallic like behavior is suggested to be predisposed by the extrinsic electrons induced by the substitutional disorder. This study further demonstrates the possibility of band gap engineering through heavy metal doping in 2D materials.",1812.00157v2 2021-05-19,Synthesis and properties of free-standing monolayer amorphous carbon,"Bulk amorphous materials have been studied extensively and are widely used, yet their atomic arrangement remains an open issue. Although they are generally believed to be Zachariasen continuous random networks, recent experimental evidence favours the competing crystallite model in the case of amorphous silicon. In two-dimensional materials, however, the corresponding questions remain unanswered. Here we report the synthesis, by laser-assisted chemical vapour deposition, of centimetre-scale, free-standing, continuous and stable monolayer amorphous carbon, topologically distinct from disordered graphene. Unlike in bulk materials, the structure of monolayer amorphous carbon can be determined by atomic-resolution imaging. Extensive characterization by Raman and X-ray spectroscopy and transmission electron microscopy reveals the complete absence of long-range periodicity and a threefold-coordinated structure with a wide distribution of bond lengths, bond angles, and five-, six-, seven- and eight-member rings. The ring distribution is not a Zachariasen continuous random network, but resembles the competing (nano)crystallite model. We construct a corresponding model that enables density-functional-theory calculations of the properties of monolayer amorphous carbon, in accordance with observations. Direct measurements confirm that it is insulating, with resistivity values similar to those of boron nitride grown by chemical vapour deposition. Free-standing monolayer amorphous carbon is surprisingly stable and deforms to a high breaking strength, without crack propagation from the point of fracture. The excellent physical properties of this stable, free-standing monolayer amorphous carbon could prove useful for permeation and diffusion barriers in applications such as magnetic recording devices and flexible electronics.",2105.08926v1 2021-07-08,Synergistic effect of workfunction and acoustic impedance mismatch for improved thermoelectric performance in GeTe/WC composite,"The preparation of composite materials is promising for concurrent optimization of electrical and thermal transport properties to realize an improved thermoelectric (TE) performance. We report the effect of work function and acoustic impedance mismatch (AIM) on the TE properties of (1-z)Ge0.87Mn0.05Sb0.08Te/(z)WC composite. In particular, a composite consisting of Mn and Sb co-doped GeTe as a matrix and WC as a dispersed phase is prepared, and its structural and TE properties are investigated. The simultaneous increase in electrical conductivity ({\sigma}) and Seebeck coefficient ({\alpha}) with WC volume fraction (z) results in an enhanced power factor ({\alpha}^2{\sigma}) in the composite. The rise in {\sigma} is attributed to increased carrier mobility in the composite. This is further established from the work function measurement using the Kelvin probe force microscopy (KPFM) technique and is also supported by the density functional theory (DFT) calculations. The difference in elastic properties (sound velocity) between Ge0.87Mn0.05Sb0.08Te and WC results in a high AIM that leads to a large interface thermal resistance (Rint) between the phases. The correlation between Rint and the Kapitza radius results in reduced phonon thermal conductivity (\kappa_ph) of the composite and is discussed using the Bruggeman asymmetrical model. The decrease in \kappa_{ph} is further established using phonon dispersion calculations that indicates the decrease in phonon group velocity in the composite. The simultaneous effect of enhanced {\alpha}^2{\sigma} and reduced \kappa_ph results in a maximum figure of merit (zT) of 1.93 at 773K for (1-z)Ge0.87Mn0.05Sb0.08Te/(z)WC composite having z=0.010. This study shows promise to achieve higher zTav across a wide range of composite materials having similar electronic structure and different elastic properties.",2107.03803v2 2022-09-09,Asymmetrical contact scaling and measurements in MoS2 FETs,"Two-dimensional (2D) materials have great potential for use in future electronics due to their atomically thin nature which withstands short channel effects and thus enables better scalability. Device scaling is the process of reducing all device dimensions to achieve higher device density in a certain chip area. For 2D materials-based transistors, both the channel and contact scalability must be investigated. The channel scalability of 2D materials has been thoroughly investigated, confirming their resilience to short-channel effects. However, systematic studies on contact scalability remain rare and the current understanding of contact scaling in 2D FET is inconsistent and oversimplified. Here we combine physically scaled contacts and asymmetrical contact measurements to investigate the contact scaling behavior in 2D field-effect transistors (FETs). The asymmetrical contact measurements directly compare electron injection with different contact lengths while using the exact same channel, eliminating channel-to-channel variations. Compared to devices with long contact lengths, devices with short contact lengths (scaled contacts) exhibit larger variation, smaller drain currents at high drain-source voltages, and a higher chance of showing early saturation and negative differential resistance. Quantum transport simulations show that the transfer length of Ni-MoS2 contacts can be as short as 5 nm. Our results suggest that charge injection at the source contact is different from injection at the drain side: scaled source contacts can limit the drain current, whereas scaled drain contacts cannot. Furthermore, we clearly identified that the transfer length depends on the quality of the metal-2D interface. The asymmetrical contact measurements proposed here will enable further understanding of contact scaling behavior at various interfaces.",2209.04144v2 2023-05-12,Disorder and cavity evolution in single-crystalline Ge during implantation of Sb ions monitored in-situ by spectroscopic ellipsometry,"Ion implantation has been a key technology for the controlled surface modification of materials in microelectronics and generally, for tribology, biocompatibility, corrosion resistance and many more. To form shallow junctions in Ge is a challenging task. In this work the formation and accumulation of shallow damage profiles was studied by in-situ spectroscopic ellipsometry (SE) for the accurate tracking and evaluation of void and damage fractions in crystalline Ge during implantation of 200-keV Sb ions with a total fluence up to 1E16 cm-2 and an ion flux of 2.1E12 cm-2 s-1. The consecutive stages of damage accumulation were identified using optical multi-layer models with quantitative parameters of the thickness of modified layers as well as the volume fractions of amorphized material and voids. The effective size of damaged zones formed from ion tracks initiated by individual bombarding ions can be estimated by numerical simulation compared with the dynamics of damage profiles measured by ion beam analysis and ellipsometry. According to our observations, the formation of initial partial disorder was followed by complete amorphization and void formation occurring at the fluence of about 1E15 cm-2, leading to a high volume fraction of voids and a modified layer thickness of approx. 200 nm by the end of the irradiation process. This agrees with the results of numerical simulations and complementary scanning electron microscopy (SEM) measurements. In addition, we found a quasi-periodic time dependent behavior of amorphization and void formation represented by alternating accelerations and decelerations of different reorganization processes, respectively.",2305.07635v1 2006-03-08,Colossal Magnetoresistance Observed in Monte Carlo Simulations of the One- and Two-Orbital Models for Manganites,"The one- and two-orbital double-exchange models for manganites are studied using Monte Carlo computational techniques in the presence of a robust electron-phonon coupling (but neglecting the antiferromagnetic exchange $J_{\rm AF}$ between the localized spins). The focus in this effort is on the analysis of charge transport. Our results for the one-orbital case confirm and extend previous recent investigations that showed the presence of robust peaks in the resistivity vs. temperature curves for this model. Quenched disorder substantially enhances the magnitude of the effect, while magnetic fields drastically reduce the resistivity. A simple picture for the origin of these results is presented. It is also shown that even for the case of just one electron, the resistance curves present metallic and insulating regions by varying the temperature, as it occurs at finite electronic density. Moreover, in the present study these investigations are extended to the more realistic two-orbital model for manganites. The transport results for this model show large peaks in the resistivity vs. temperature curves, located at approximately the Curie temperature, and with associated large magnetoresistance factors. Overall, the magnitude and shape of the effects discussed here closely resemble experiments for materials such as $\rm La_{0.70} Ca_{0.30} Mn O_{3}$, and they are in qualitative agreement with the current predominant theoretical view that competition between a metal and an insulator, enhanced by quenched disorder, is crucial to understand the colossal magnetoresistance (CMR) phenomenon.",0603221v1 2017-11-02,Non-equilibrium character of resistive switching and negative differential resistance in Ga-doped Cr2O3 system,"We have synthesized Ga-doped Cr2O3 system with compositions Cr1.45Ga0.55O3 and Cr1.17Ga0.83O3 by chemical co-precipitation route and post annealing at 800^C. The samples have been stabilized in rhombohedral crystal structure with space group R3C. The present work focuses on the study of non-linear current-voltage (I-V) characteristics of the samples, which exhibited many interesting electronic properties, e.g., I-V loop, resistive switching, bi-stable electronic states, and negative differential resistance. The non-equilibrium character of the I-V characteristics has been studied by measurement of bias voltage cycling up to 20 times and current relaxation with time at set bias voltage. The charge conduction process in the samples has been understood by analysing I-V curves using different phenomenological models based on electrode-limited and bulk-limited charge conduction mechanisms proposed for metal electrode-metal oxide-metal electrode (M-MO-M) junctions. It is understood that competitions between injection of charge carriers from metal electrode to metal oxide, charge flow through the material (trapping/de-trapping and recombination of charge carriers at the defect sites), space charge formation at the junctions of electrodes and metal oxides, and ejection of electrons from metal oxide to metal electrode control the non-equilibrium I-V characteristics in the present samples.",1711.00687v1 2020-04-24,Graphene-Polyurethane Coatings for Deformable Conductors and Electromagnetic Interference Shielding,"Electrically conductive, polymeric materials that maintain their conductivity even when under significant mechanical deformation are needed for actuator electrodes, conformable electromagnetic shielding, stretchable tactile sensors and flexible energy storage. The challenge for these materials is that the percolated, electrically conductive networks tend to separate even at low strains, leading to significant piezoresistance. Herein, deformable conductors were fabricated by spray-coating a nitrile substrate with a graphene-elastomer solution. The coatings showed only slight increase in electrical resistance after thousands of bending cycles and repeated folding-unfolding events. The deformable conductors doubled their electrical resistance at 12% strain and were washable without changing their electrical properties. The conductivity-strain behaviour was modelled by considering the nanofiller separation upon deformation. To boost the conductivity at higher strains, the production process was adapted by stretching the nitrile substrate before spraying, after which it was released. This adaption meant that the electrical resistance doubled at 25 % strain. The electrical resistance was found sufficiently low to give a 1.9 dB/{\mu}m shielding in the 8-12 GHz electromagnetic band. The physical and electrical properties, including the EM screening, of the flexible conductors, were found to deteriorate upon cycling but could be recovered through reheating the coating.",2004.11613v1 2016-03-20,Three-dimensional resistivity switching between correlated electronic states in 1T-TaS2,"Recent demonstrations of controlled switching between different ordered macroscopic states by impulsive electromagnetic perturbations in complex materials have opened some fundamental questions on the mechanisms responsible for such remarkable behavior. Here we experimentally address the question of whether two-dimensional (2D) Mott physics can be responsible for unusual switching between states of different electronic order in the layered dichalcogenide 1T-TaS2, or it is a result of subtle inter-layer orbitronic re-ordering of its helical stacking structure. We report on the switching properties both in-plane and perpendicular to the layers by current-pulse injection, the anisotropy of electronic transport in the commensurate ground state, and relaxation properties of the switched metastable state. Contrary to recent theoretical calculations, which predict a uni-directional metal perpendicular to the layers, we observe a large resistivity in this direction, with a temperature-dependent anisotropy. Remarkably, large resistance ratios are observed in the memristive switching both in-plane (IP) and out-of-plane (OP). The relaxation dynamics of the metastable state for both IP and OP electron transport are seemingly governed by the same mesoscopic quantum re-ordering process. We conclude that 1T-TaS2 shows resistance switching arising from an interplay of both IP and OP correlations.",1603.06214v1 2019-12-17,Antiferromagnetic CuMnAs: Ab initio description of finite temperature magnetism and resistivity,"Noncollinear magnetic moments in antiferromagnets (AFM) lead to a complex behavior of electrical transport, even to a decreasing resistivity due to an increasing temperature. Proper treatment of such phenomena is required for understanding AFM systems at finite temperatures; however first-principles description of these effects is complicated. With ab initio techniques, we investigate three models of spin fluctuations (magnons) influencing the transport in AFM CuMnAs; the models are numerically feasible and easily implementable to other studies. We numerically justified a fully relativistic collinear disordered local moment approach and we present its uncompensated generalization. A saturation or a decrease of resistivity caused by magnons, phonons, and their combination (above approx. 400 K) was observed and explained by changes in electronic structure. Within the coherent potential approximation, our finite-temperature approaches may be applied also to systems with impurities, which are found to have a large impact not only on residual resistivity, but also on canting of magnetic moments from the AFM to the ferromagnetic (FM) state.",1912.08025v4 2020-12-30,Non-thermal light-assisted resistance collapse in a V$_2$O$_3$-based Mott-insulator device,"The insulator-to-metal transition in Mott insulators is the key mechanism for a novel class of electronic devices, belonging to the Mottronics family. Intense research efforts are currently devoted to the development of specific control protocols, usually based on the application of voltage, strain, pressure and light excitation. The ultimate goal is to achieve the complete control of the electronic phase transformation, with dramatic impact on the performance, for example, of resistive switching devices. Here, we investigate the simultaneous effect of external voltage and excitation by ultrashort light pulses on a single Mottronic device based on a V$_2$O$_3$ epitaxial thin film. The experimental results, supported by finite-element simulations of the thermal problem, demonstrate that the combination of light excitation and external electrical bias drives a volatile resistivity drop which goes beyond the combined effect of laser and Joule heating. Our results impact on the development of protocols for the non-thermal control of the resistive switching transition in correlated materials.",2012.15255v2 2023-06-07,Slip Resistance Test Apparatus of Synthetic Rubber Trackpad on Photovoltaic Surface,"The increasing development of the solar energy industry in many countries has led to a rising frequency of human and robot presence in this area. To ensure occupational safety, various protective equipment, including rubber material, is commonly used for slip resistance while moving on the surface of solar PV panels. Therefore, the slip resistance test apparatus is built for testing the slip resistance between the synthetic rubber trackpad and the photovoltaic panel (PV) surface. Synthetic rubber is a man-made material, so it is difficult to control the parameters of its mechanical and chemical properties absolutely. Variations in wet/dry working conditions or Shore hardness are factors that make slip computation more challenging. Therefore, an apparatus with the principle of converting the reciprocating motion of the screw and the casters into the rotation of the hinge is introduced to adjust the tilt angle of the upper surface, detect and evaluate the slippage of the rubber trackpad by sensors. Some parameters related to accuracy such as vibration and theoretical-empirical assessment, are also mentioned. In addition to designing a reliable apparatus, the article also succeeded in providing a safety standard for synthetic rubber with Shore A30-A40 when moving on PV surfaces.",2306.10032v1 2023-08-14,Temperature-dependent $f$-electron evolution in CeCoIn$_5$ via a comparative infrared study with LaCoIn$_5$,"We investigated CeCoIn$_5$ and LaCoIn$_5$ single crystals, which have the same HoCoGa$_5$-type tetragonal crystal structure, using infrared spectroscopy. However, while CeCoIn$_5$ has 4$f$ electrons, LaCoIn$_5$ does not. By comparing these two material systems, we extracted the temperature-dependent electronic evolution of the $f$ electrons of CeCoIn$_5$. We observed that the differences caused by the $f$ electrons are more obvious in low-energy optical spectra at low temperatures. We introduced a complex optical resistivity and obtained a magnetic optical resistivity from the difference in the optical resistivity spectra of the two material systems. From the temperature-dependent average magnetic resistivity, we found that the onset temperature of the Kondo effect is much higher than the known onset temperature of Kondo scattering ($\simeq$ 200 K) of CeCoIn$_5$. Based on momentum-dependent hybridization, the periodic Anderson model, and a maximum entropy approach, we obtained the hybridization gap distribution function of CeCoIn$_5$ and found that the resulting gap distribution function of CeCoIn$_5$ was mainly composed of two (small and large) components (or gaps). We assigned the small and large gaps to the in-plane and out-of-plane hybridization gaps, respectively. We expect that our results will provide useful information for understanding the temperature-dependent electronic evolution of $f$-electron systems near Fermi level.",2308.06881v1 2024-02-01,Mott resistive switching initiated by topological defects,"Resistive switching is the fundamental process that triggers the sudden change of the electrical properties in solid-state devices under the action of intense electric fields. Despite its relevance for information processing, ultrafast electronics, neuromorphic devices, resistive memories and brain-inspired computation, the nature of the local stochastic fluctuations that drive the formation of metallic nuclei out of the insulating state has remained hidden. Here, using operando X-ray nano-imaging, we have captured the early-stages of resistive switching in a V2O3-based device under working conditions. V2O3 is a paradigmatic Mott material, which undergoes a first-order metal-to-insulator transition coupled to a lattice transformation that breaks the threefold rotational symmetry of the rhombohedral metal phase. We reveal a new class of volatile electronic switching triggered by nanoscale topological defects of the lattice order parameter of the insulating phase. Our results pave the way to the use of strain engineering approaches to manipulate topological defects and achieve the full control of the electronic Mott switching. The concept of topology-driven reversible electronic transition is of interest for a broad class of quantum materials, comprising transition metal oxides, chalcogenides and kagome metals, that exhibit first-order electronic transitions coupled to a symmetry-breaking order.",2402.00747v1 2024-05-14,"A new ferromagnetic semiconductor system of Eu$_{1-x}$Sr$_x$AgP $(x = 0.0-0.6)$ compounds: Crystallographic, magnetic, and magneto-resistive properties","Adjusting chemical pressure through doping is a highly effective method for customizing the chemical and physical properties of materials, along with their respective phase diagrams, thereby uncovering novel quantum phenomena. Here, we successfully synthesized Sr-doped Eu$_{1-x}$Sr$_x$AgP $(x = 0.0-0.6)$ and conducted a comprehensive investigation involving crystallography, magnetization, heat capacity, and magnetoresistance. Utilizing X-ray diffraction and PPMS DynaCool measurements, we studied Eu$_{1-x}$Sr$_x$AgP in detail. The hexagonal structure of parent EuAgP at room temperature, with the $P6_3/mmc$ space group, remains unaltered, while the lattice constants expand. The magnetic phase transition from paramagnetism to ferromagnetism, as temperature decreases, is suppressed through the gradual introduction of strontium doping. Heat capacity measurements reveal a shift from magnon-dominated to predominantly phonon and electron contributions near the ferromagnetic phase with increasing doping levels. The resistivity-temperature relationship displays distinct characteristics, emphasizing the impact of Sr doping on modifying charge transport. Magnetoresistance measurements uncover novel phenomena, illustrating the adjustability of magnetoresistance through Sr doping. Notably, Sr doping results in both positive magnetoresistance (up to 20\%) and negative magnetoresistance (approximately -60\%). The resistivity and magnetic phase diagram were established for the first time, revealing the pronounced feasibility of Sr doping in modulating EuAgP's resistivity. This study has provided valuable insights into the intricate interplay between structural modifications and diverse physical properties. The potential for technological advancements and the exploration of novel quantum states make Sr-doped Eu$_{1-x}$Sr$_x$AgP a compelling subject for continued research in the field of applied physics.",2405.08357v1 1999-04-01,Radio-frequency impedance measurements using a tunnel-diode oscillator (TDO) technique,"A resonant method based on a tunnel-diode oscillator (TDO) for precision measurements of relative impedance changes in materials, is described. The system consists of an effective self-resonant LC-tank circuit driven by a forward-biased tunnel diode operating in its negative resistance region. Samples under investigation are placed in the core of an inductive coil and impedance changes are determined directly from the measured shift in resonance frequency. A customized low temperature insert is used to integrate this experiment with a commercial Model 6000 Physical Property Measurement System (Quantum Design). Test measurements on a manganese-based perovskite sample exhibiting colossal magneto-resistance (CMR) indicate that this method is well suited to study the magneto-impedance in these materials.",9904026v1 2000-01-19,Pseudogap effects on the c-axis charge dynamics in copper oxide materials,"The c-axis charge dynamics of copper oxide materials in the underdoped and optimally doped regimes has been studied by considering the incoherent interlayer hopping. It is shown that the c-axis charge dynamics for the chain copper oxide materials is mainly governed by the scattering from the in-plane fluctuation, and the c-axis charge dynamics for the no-chain copper oxide materials is dominated by the scattering from the in-plane fluctuation incorporating with the interlayer disorder, which would be suppressed when the holon pseudogap opens at low temperatures and lower doping levels, leading to the crossovers to the semiconducting-like range in the c-axis resistivity and the temperature linear to the nonlinear range in the in-plane resistivity.",0001260v1 2002-02-27,Anisotropic Magnetoresistance in Ga$_{1-x}$Mn$_x$As,"We have measured the magnetoresistance in a series of Ga$_{1-x}$Mn$_x$As samples with 0.033$\le x \le$ 0.053 for three mutually orthogonal orientations of the applied magnetic field. The spontaneous resistivity anisotropy (SRA) in these materials is negative (i.e. the sample resistance is higher when its magnetization is perpendicular to the measuring current than when the two are parallel) and has a magnitude on the order of 5% at temperatures near 10K and below. This stands in contrast to the results for most conventional magnetic materials where the SRA is considerably smaller in magnitude for those few cases in which a negative sign is observed. The magnitude of the SRA drops from its maximum at low temperatures to zero at T$_C$ in a manner that is consistent with mean field theory. These results should provide a significant test for emerging theories of transport in this new class of materials.",0202508v1 2008-05-28,Unified explanation of the Kadowaki-Woods ratio in strongly correlated materials,"Discoveries of ratios whose values are constant within broad classes of materials have led to many deep physical insights. The Kadowaki-Woods ratio (KWR) compares the temperature dependence of a metal's resistivity to that of its heat capacity; thereby probing the relationship between the electron-electron scattering rate and the renormalisation of the electron mass. However, the KWR takes very different values in different materials. Here we introduce a ratio, closely related to the KWR, that includes the effects of carrier density and spatial dimensionality and takes the same (predicted) value in organic charge transfer salts, transition metal oxides, heavy fermions and transition metals - despite the numerator and denominator varying by ten orders of magnitude. Hence, in these materials, the same emergent physics is responsible for the mass enhancement and the quadratic temperature dependence of the resistivity and no exotic explanations of their KWRs are required.",0805.4275v4 2016-06-15,Suppression of lattice thermal conductivity by mass-conserving cation mutation in multi-component semiconductors,"In semiconductors almost all heat is conducted by phonons (lattice vibrations), which is limited by their quasi-particle lifetimes. Phonon-phonon interactions represent scattering mechanisms that produce thermal resistance. In thermoelectric materials, this resistance due to anharmonicity should be maximised for optimal performance. We use a first-principles lattice-dynamics approach to explore the changes in lattice dynamics across an isostructural series where the average atomic mass is conserved: ZnS to CuGaS$_2$ to Cu$_2$ZnGeS$_4$. Our results demonstrate an enhancement of phonon interactions in the multernary materials, and confirm that lattice thermal conductivity can be controlled independently of the average mass and local coordination environments.",1606.04914v1 2018-06-12,Determination of the BCS material parameters of the HIE-ISOLDE superconducting resonator,"Superconducting material parameters of the Nb film coating on the Quarter-Wave Resonator (QWR) for the HIE-ISOLDE project were studied by fitting experimental results with the Mattis-Bardeen theory. We pointed out a strong correlation among fitted estimators of material parameters in the BCS theory, and proposed a procedure to remove the correlation by simultaneously fitting the surface resistance and effective penetration depth. Unlike previous studies, no literature values were assumed in the fitting. As surface resistance and penetration depth had a similar dependence on coherence length and mean free path, the correlation between these two parameters could not be eliminated by this fitting. The upper critical field measured by SQUID magnetometry showed complementary constraint to the RF result, and this allowed all the material parameters to be determined.",1806.04443v1 2018-09-19,Electrical Parameters for Planar Transport in Graphene and 2-D Materials,"Classical electrodynamics has been revisited with a view to recast the electrical parameters for planar transport in 2-dimensional (2-D) materials like graphene. In this attempt a new line integral, named transverse line integral, with extensive applications in 2-D, is defined. Since the existing divergence theorem in not applicable in 2-D, we introduced a new divergence theorem. A new definition for the in-plane flux of any 2-D vector is introduced. A new vector named electric vector potential is defined and Gauss law is modified in terms of the 2-D flux of the new vector. The new Gauss law in presence of dielectric is obtained and a new electric displacement vector is defined for the 2-D materials. The conduction and displacement current densities in 2-D are defined. Resistance and resistivity in 2-D materials are discussed. The continuity equation for planar transport is derived.",1809.07319v1 2020-09-04,Fracture mechanics of micro samples: Fundamental considerations,"In this review article we consider the crack growth resistance ofmicrometer and submicrometer sized samples from the fracture mechanics point of view. Standard fracture mechanics test procedures were developed for macroscale samples, and reduction of the specimen dimensions by three to five orders of magnitude has severe consequences. This concerns the interpretation of results obtained by micro and nanomechanics, as well as the life time and failure prediction of micro and nano devices. We discuss the relevant fracture mechanics length scales and their relation to the material specific structural lengths in order to conduct rigorous fracture mechanics experiments. To ensure general validity and applicability of evaluation concepts, these scaling considerations are detailed for ideally brittle, semi brittle and micro ductile crack propagation, subject to both monotonic and cyclic loading. Special attention is devoted to the requirements for determining specimen size for various loading types to measure material characteristic crack propagation resistance at small scales. Finally, we discuss novel possibilities of micron and submicron fracture mechanics tests to improve the basic understanding of specific crack propagation processes.",2009.05386v1 2015-07-23,Ba{0.4}Rb{0.6}Mn2As2: A Prototype Half-Metallic Ferromagnet,"Half-metallic ferromagnetism (FM) in single-crystal Ba{0.39(1)}Rb{0.61(1)}Mn2As2 below its Curie temperature TC = 103(2) K is reported. The magnetization M versus applied magnetic field H isotherm data at 1.8 K show complete polarization of the itinerant doped-hole magnetic moments that are introduced by substituting Rb for Ba. The material exhibits extremely soft FM, with unobservably small remanent magnetization and coercive field. Surprisingly, and contrary to typical itinerant FMs, the M(H) data follow the Arrott-plot paradigm that is based on a mean-field theory of local-moment FMs. The in-plane electrical resistivity data are fitted well by an activated-T^2 expression for T < TC, whereas the data sharply deviate from this model for T > TC. Hence the activated-T^2 resistivity model is an excellent diagnostic for determining the onset of half-metallic FM in this compound, which in turn demonstrates the presence of a strong correlation between the electronic transport and magnetic properties of the material. Together with previous data on 40% hole-doped Ba{0.6}K{0.4}Mn2As2, these measurements establish 61%-doped Ba{0.39}Rb{0.61}Mn2As2 as a prototype for a new class of half-metallic ferromagnets in which all the itinerant carriers in the material are ferromagnetic.",1507.06679v1 2018-12-18,Atomistic study of an ideal metal/thermoelectric contact: the full-Heusler/half-Heusler interface,"Half-Heusler alloys such as the (Zr,Hf)NiSn intermetallic compounds are important thermoelectric materials for converting waste heat into electricity. Reduced electrical resistivity at the hot interface between the half-Heusler material and a metal contact is critical for device performance, however this has yet to be achieved in practice. Recent experimental work suggests that a coherent interface between half-Heusler and full-Heusler compounds can form due to diffusion of transition metal atoms into the vacant sublattice of the half-Heusler lattice. We study theoretically the structural and electronic properties of such an interface using a first-principles based approach that combines {\it ab initio} calculations with macroscopic modeling. We find that the prototypical interface HfNi$_2$Sn/HfNiSn provides very low contact resistivity and almost ohmic behavior over a wide range of temperatures and doping levels. Given the potential of these interfaces to remain stable over a wide range of temperatures, our study suggests that full-Heuslers might provide nearly ideal electrical contacts to half-Heuslers that can be harnessed for efficient thermoelectric generator devices.",1812.07189v1 2020-11-21,All-Materials-Inclusive Flash Spark Plasma Sintering,"A new flash (ultra-rapid) spark plasma sintering method applicable to various materials systems, regardless of their electrical resistivity, is developed. A number of powders ranging from metals to electrically insulative ceramics have been successfully densified resulting in homogeneous microstructures within sintering times of 8-35 s. A finite element simulation reveals that the developed method, providing an extraordinary fast and homogeneous heating concentrated in the sample's volume and punches, is applicable to all the different samples tested. The utilized uniquely controllable flash phenomenon is enabled by the combination of the electric current concentration around the sample and the confinement of the heat generated in this area by the lateral thermal contact resistance. The presented new method allows: extending flash sintering to nearly all materials, controlling sample shape by an added graphite die, and an energy efficient mass production of small and intermediate size objects. This approach represents also a potential venue for future investigations of flash sintering of complex shapes.",2011.14012v1 2021-03-26,A micropolar continuum model of diffusion creep,"Solid polycrystalline materials undergoing diffusion creep are usually described by Cauchy continuum models with a Newtonian viscous rheology dependent on the grain size. Such a continuum lacks the rotational degrees of freedom needed to describe grain rotation. Here we provide a more general continuum description of diffusion creep that includes grain rotation, and identifies the deformation of the material with that of a micropolar (Cosserat) fluid. We derive expressions for the micropolar constitutive tensors by a homogenisation of the physics describing a discrete collection of rigid grains, demanding an equivalent dissipation between the discrete and continuum descriptions. General constitutive laws are derived for both Coble (grain-boundary diffusion) and Nabarro-Herring (volume diffusion) creep. Detailed calculations are performed for a two-dimensional tiling of irregular hexagonal grains, which illustrates a potential coupling between the rotational and translational degrees of freedom. If only the plating out or removal of material at grain boundaries is considered, the constitutive laws are degenerate: modes of deformation that involve pure tangential motion at the grain boundaries are not resisted. This degeneracy can be removed by including the resistance to grain-boundary sliding, or by imposing additional constraints on the deformation.",2103.14458v3 2021-04-30,Material surface -- analyte interactions with similar energy rates vary as univariate quadratic function of topological polar surface area of analytes,"Material surface - analyte interactions play important roles in numerous processes including gas sensing. However, the effects of topological polar surface area (TPSA) of analytes on surface interactions during gas sensing have been so far largely disregarded. In this work, based on experimental observations on changes in electrical resistance of cadmium sulphide (CdS) due to surface interactions during gas sensing, we found that unexpected univariate quadratic correlation exists between changes in resistance of CdS and TPSA of analytes. Further experiments on four other material systems showed the same trend, revealing a generalized picture of TPSA dependence of surface interactions.",2104.14867v1 2022-06-08,Scalable fabrication of edge contacts to 2D materials,"We present a fabrication method for reliably and reproducibly forming electrical contacts to 2D materials, based on the tri-layer resist system. We demonstrate the applicability of this method for epitaxial graphene on silicon carbide (epigraphene) and the transition metal dichalcogenides (TMDCs) molybdenum disulfide ($MoS_2$). For epigraphene, the specific contact resistances are of the order of $\rho_c$ ~ $50$ $\Omega\mu m$, and follow the Landauer quantum limit, $\rho_c \propto n^{-1/2}$, with $n$ being the carrier density of graphene. For $MoS_2$ flakes, our edge contacts enable field effect transistors (FET) with ON/OFF ratio of $> 10^6$ at room temperature ( $> 10^9$ at cryogenic temperatures). The fabrication route here demonstrated allows for contact metallization using thermal evaporation and also by sputtering, giving an additional flexibility when designing electrical interfaces, which is key in practical devices and when exploring the electrical properties of emerging materials.",2206.03839v2 2022-07-04,An Important Structural Requirement for the Superconductor Material: A Hypothesis,"On a microscopic scale, resistivity during electric conduction is caused by collisions of the free conduction electrons with the obstructing atoms or molecules of the conductor material, resulting in heat production. Based on this fundamental understanding, a hypothesis concerning a physical requirement of the superconductor material is proposed, which suggests that for superconductivity (i.e., with zero resistivity) to occur, the conductor material must have nano-sized, continuous and straight vacuum tunnels inside with effective radius size large enough to allow collision-free conduction of free electrons. Besides, some of the composite atoms of the conductor should be able to readily release electrons to form the conduction band; in fact, this basic requirement is for all forms of electrical conductors, not just for superconductors. The proposed hypothesis is supported by experimental observations in the literature, and also offers a plausible explanation for some of the poorly-understood experimental phenomena observed in the past. In addition, the hypothesis offers practical strategies for the rational design of electrical conductors with (quasi-)superconductivity. Lastly, the proposed new hypothesis also suggests a novel mechanism for neural microtubule-mediated electrical quasi-superconductance in the nervous system.",2207.01226v2 1994-06-03,"Localization Effects in Bi2Sr2Ca(Cu,Co)2O8+y High Temperature Superconductors","Doping Bi2Sr2Ca1Cu2O8+y with Co causes a superconductor-insulator transition. We study correlations between changes in the electrical resistivity RHOab(T) and the electronic bandstructure using identical single crystalline samples. For undoped samples the resistivity is linear in temperature and has a vanishing residual resistivity. In angle resolved photoemission these samples show dispersing band-like states. Co-doping decreases TC and causes and increase in the residual resistivity. Above a threshold Co-concentration the resistivity is metallic (drab/dT >0) at room temperature, turns insulating below a characteristic temperature Tmin and becomes super- conducting at even lower temperature. These changes in the resistivity correlate with the disappearance of the dispersing band-like states in angle resolved photoemission. We show that Anderson localization caused by the impurity potential of the doped Co-atoms provides a consistent explanation of all experimental features. Therefore the TC reduction in 3d-metal doped high- temperature superconductors is not caused by Abrikosov Gor'kov pair- breaking but by spatial localization of the carriers. The observed suppression of TC indicates that the system is in the homogenous limit of the superconductor-insulator transition. The coexistance of insulating (dRHOab/dT <0) normal state behavior and super- conductivity indicates that the superconducting ground state is formed out of spatially almost localized carriers.",9406021v1 2011-11-17,Stability of a self-gravitating homogeneous resistive plasma,"In this paper, we analyze the stability of a homogeneous self-gravitating plasma, having a non-zero resistivity. This study provides a generalization of the Jeans paradigm for determining the critical scale above which gravitational collapse is allowed. We start by discussing the stability of an ideal self-gravitating plasma embedded in a constant magnetic field. We outline the existence of an anisotropic feature of the gravitational collapse. In fact, while in the plane orthogonal to the magnetic field the Jeans length is enhanced by the contribution of the magnetic pressure, outside this plane perturbations are governed by the usual Jeans criterium. The anisotropic collapse of a density contrast is sketched in details, suggesting that the linear evolution provides anisotropic initial conditions for the non-linear stage, where this effect could be strongly enforced. The same problem is then faced in the presence of non-zero resistivity and the conditions for the gravitational collapse are correspondingly extended. The relevant feature emerging in this resistive scenario is the cancellation of the collapse anisotropy in weakly conducting plasmas. In this case, the instability of a self-gravitating resistive plasma is characterized by the standard isotropic Jeans length in any directions. The limit of very small resistivity coefficient is finally addressed, elucidating how reminiscence of the collapse anisotropy can be found in the different value of the perturbation frequency inside and outside the plane orthogonal to the magnetic field.",1111.4051v1 2013-02-26,Inter-plane resistivity of isovalent doped BaFe$_2$(As$_{1-x}$P$_x$)$_2$,"Temperature-dependent inter-plane resistivity, $\rho_c(T)$, was measured for the iron-based superconductor BaFe$_2$(As$_{1-x}$P$_x$)$_2$ over a broad isoelectron phosphorus substitution range from $x$=0 to $x$=0.60, from non-superconducting parent compound to heavily overdoped superconducting composition with $T_c\approx 10 K$. The features due to structural and magnetic transitions are clearly resolved in $\rho_c(T)$ of the underdoped crystals. A characteristic maximum in $\rho_c(T)$, found in the parent BaFe$_2$As$_2$ at around 200 K, moves rapidly with phosphorus substitution to high temperatures. At the optimal doping, the inter-plane resistivity shows $T$-linear temperature dependence without any cross-over anomalies, similar to the previously reported in-plane resistivity. This observation is in stark contrast with dissimilar temperature dependences found at optimal doping in electron-doped Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$. Our finding suggests that despite similar values of the resistivity and its anisotropy, the temperature dependent transport in the normal state is very different in electron and isoelectron doped compounds. Similar temperature dependence of both in-plane and inter-plane resistivities, in which the dominant contributions are coming from different parts of the Fermi surface, suggests that scattering is the same on the whole Fermi surface. Since magnetic fluctuations are expected to be much stronger on the quasi-nested sheets, this observation may point to the importance of the inter-orbital scattering between different sheets.",1302.6440v1 2013-05-16,Effect of doping on the magnetostructural ordered phase of iron arsenides: A comparative study of the resistivity anisotropy in the doped BaFe$_2$As$_2$ with doping into three different sites,"In order to unravel a role of doping in the iron-based superconductors, we investigated the in-plane resistivity for BaFe$_2$As$_2$ doped at either of the three different lattice sites, Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$, BaFe$_2$(As$_{1-x}$P$_x$)$_2$, and Ba$_{1-x}$K$_x$Fe$_2$As$_2$, focusing on the doping effect in the low-temperature antiferromagnetic/orthorhombic (AFO) phase. A major role of doping in the high-temperature paramagnetic/tetragonal (PT) phase is known to change the Fermi surface by supplying charge carriers or by exerting chemical pressure. In the AFO phase, we found a clear correlation between the magnitude of residual resistivity and resistivity anisotropy. This indicates that the resistivity anisotropy originates from the anisotropic impurity scattering from dopant atoms. The magnitude of residual resistivity is also found to be a parameter controlling the suppression rate of AFO ordering temperature $T_s$. Therefore, the dominant role of doping in the AFO phase is to introduce disorder to the system, distinct from that in the PT phase.",1305.3744v1 2016-01-13,Limiting the Development of Anti-Cancer Drug Resistance in a Spatial Model of Micrometastases,"While chemoresistance in primary tumors is well-studied, much less is known about the influence of systemic chemotherapy on the development of drug resistance at metastatic sites. In this work, we use a hybrid spatial model of tumor response to a DNA damaging drug to study how the development of chemoresistance in micrometastases depends on the drug dosing schedule. We separately consider cell populations that harbor pre-existing resistance to the drug, and those that acquire resistance during the course of treatment. For each of these independent scenarios, we consider one hypothetical cell line that is responsive to metronomic chemotherapy, and another that with high probability cannot be eradicated by a metronomic protocol. Motivated by experimental work on ovarian cancer xenografts, we consider all possible combinations of a one week treatment protocol, repeated for three weeks, and constrained by the total weekly drug dose. Simulations reveal a small number of fractionated-dose protocols that are at least as effective as metronomic therapy in eradicating micrometastases with acquired resistance (weak or strong), while also being at least as effective on those that harbor weakly pre-existing resistant cells. Given the responsiveness of very different theoretical cell lines to these few fractionated-dose protocols, these may represent more effective ways to schedule chemotherapy with the goal of limiting metastatic tumor progression.",1601.03412v2 2014-01-08,Angular and Polarization Response of Multimode Sensors with Resistive-Grid Absorbers,"High sensitivity receiver systems with near ideal polarization sensitivity are highly desirable for development of millimeter and sub-millimeter radio astronomy. Multimoded bolometers provide a unique solution to achieve such sensitivity, for which hundreds of single-mode sensors would otherwise be required. The primary concern in employing such multimoded sensors for polarimetery is the control of the polarization systematics. In this paper, we examine the angular- and polarization- dependent absorption pattern of a thin resistive grid or membrane, which models an absorber used for a multimoded bolometer. The result shows that a freestanding thin resistive absorber with a surface resistivity of \eta/2, where \eta\ is the impedance of free space, attains a beam pattern with equal E- and H-plane responses, leading to zero cross polarization. For a resistive-grid absorber, the condition is met when a pair of grids is positioned orthogonal to each other and both have a resistivity of \eta/2. When a reflective backshort termination is employed to improve absorption efficiency, the cross-polar level can be suppressed below -30 dB if acceptance angle of the sensor is limited to <60degrees. The small cross-polar systematics have even-parity patterns and do not contaminate the measurements of odd-parity polarization patterns, for which many of recent instruments for cosmic microwave background are designed. Underlying symmetry that suppresses these cross-polar systematics is discussed in detail. The estimates and formalism provided in this paper offer key tools in the design consideration of the instruments using the multimoded polarimeters.",1401.1859v1 2021-08-30,Clonal Diversity at Cancer Recurrence,"Despite initial success, cancer therapies often fail due to the emergence of drug-resistant cells. In this study, we use a mathematical model to investigate how cancer evolves over time, specifically focusing on the state of the tumor when it recurs after treatment. We use a two-type branching process to capture the dynamics of both drug-sensitive and drug-resistant cells. We analyze the clonal diversity of drug-resistant cells at the time of cancer recurrence, which is defined as the first time the population size of drug-resistant cells exceeds a specified proportion of the initial population size of drug-sensitive cells. We examine two clonal diversity indices: the number of clones and the Simpson's Index. We calculate the expected values of these indices and utilize them to develop statistical methods for estimating model parameters. Additionally, we examine these two indices conditioned on early recurrence in the special case of a deterministically decaying sensitive population, with the aim of addressing the question of whether early recurrence is driven by a single mutation that generates an unusually large family of drug-resistant cells (corresponding to a low clonal diversity), or if it is due to the presence of an unusually large number of mutations causing drug resistance (corresponding to a high clonal diversity). Our findings, based on both indices, support the latter possibility. Furthermore, we demonstrate that the time of cancer recurrence can serve as a valuable indicator of clonal diversity, offering new insights for the treatment of recurrent cancers.",2108.13472v3 2022-03-23,A Fast Diagnostic to Inform Screening of Discarded or Retired Batteries,"With the increased pervasiveness of Lithium-ion batteries, there is growing concern for the amount of retired batteries that will be entering the waste stream. Although these batteries no longer meet the demands of their first application, many still have a significant portion of their initial capacity remaining for use in secondary applications. Yet, direct repurposing is generally not possible and each cell in a battery must be evaluated, increasing the cost of the repurposed packs due to the time intensive screening process. In this paper, a rapid assessment of the internal resistance of a cell is proposed. First, this method of measuring the resistance is completed on cells from twelve retired battery packs and one fresh pack using a hybrid pulse power characterization (HPPC) test as a benchmark for the analysis. Results from these tests show relatively constant resistance measurements across mid to high terminal voltages, allowing this metric to be independent of state of charge (SOC). Then, the relation between internal resistance and capacity across the various packs is discussed. Initial experimental results from this study show a correlation between internal resistance and capacity which can be approximated with a linear fit, suggesting internal resistance measurements taken above a threshold cell terminal voltage may be a suitable initial screening metric for the capacity of retired cells without knowledge of the SOC.",2203.12376v1 2023-01-15,Effects of quantum recoil forces in resistive switching in memristors,"Memristive devices, whose resistance can be controlled by applying a voltage and further retained, are attractive as possible circuit elements for neuromorphic computing. This new type of devices poses a number of both technological and theoretical challenges. Even the physics of the key process of resistive switching, usually associated with formation or breakage of conductive filaments in the memristor, is not completely understood yet. This work proposes a new resistive switching mechanism, which should be important in the thin-filament regime and take place due to the back reaction, or recoil, of quantum charge carriers -- independently of the conventional electrostatically-driven ion migration. Since thinnest conductive filaments are in question, which are only several atoms thick and allow for a quasi-ballistic, quantized conductance, we use a mean-field theory and the framework of nonequilibrium Green's functions to discuss the electron recoil effect for a quantum current through a nanofilament on its geometry and compare it with the transmission probability of charge carriers. Namely, we first study an analytically tractable toy model of a 1D atomic chain, to qualitatively demonstrate the importance of the charge-carrier recoil, and further proceed with a realistic molecular-dynamics simulation of the recoil-driven ion migration along a copper filament and the resulting resistive switching. The results obtained are expected to add to the understanding of resistive switching mechanisms at the nanoscale and to help downscale high-retention memristive devices.",2301.06066v2 2024-01-16,Resistively controlled primordial magnetic turbulence decay,"Magnetic fields generated in the early Universe undergo turbulent decay during the radiation-dominated era. The decay is governed by a decay exponent and a decay time. It has been argued that the latter is prolonged by magnetic reconnection, which depends on the microphysical resistivity and viscosity. Turbulence, on the other hand, is not usually expected to be sensitive to microphysical dissipation, which affects only very small scales. We want to test and quantify the reconnection hypothesis in decaying hydromagnetic turbulence. We performed high-resolution numerical simulations with zero net magnetic helicity using the Pencil Code with up to $2048^3$ mesh points and relate the decay time to the Alfv\'en time for different resistivities and viscosities. The decay time is found to be longer than the Alfv\'en time by a factor that increases with increasing Lundquist number to the 1/4 power. The decay exponent is as expected from the conservation of the Hosking integral, but a timescale dependence on resistivity is unusual for developed turbulence and not found for hydrodynamic turbulence. In two dimensions, the Lundquist number dependence is shown to be leveling off above values of $\approx25,000$, independently of the value of the viscosity. Our numerical results suggest that resistivity effects have been overestimated in earlier work. Instead of reconnection, it may be the magnetic helicity density in smaller patches that is responsible for the resistively slow decay. The leveling off at large Lundquist number cannot currently be confirmed in three dimensions.",2401.08569v3 2015-09-11,Model of Flux Trapping in Cooling Down Process,"The flux trapping that occurs in the process of cooling down of the superconducting cavity is studied. The critical fields $B_{c2}$ and $B_{c1}$ depend on a position when a material temperature is not uniform. In a region with $T\simeq T_c$, $B_{c2}$ and $B_{c1}$ are strongly suppressed and can be smaller than the ambient magnetic field, $B_a$. A region with $B_{c2}\le B_a$ is normal conducting, that with $B_{c1}\le B_a < B_{c2}$ is in the vortex state, and that with $B_{c1}> B_a$ is in the Meissner state. As a material is cooled down, these three domains including the vortex state domain sweep and pass through the material. In this process, vortices contained in the vortex state domain are trapped by pinning centers distributing in the material. A number of trapped fluxes can be evaluated by using the analogy with the beam-target collision event, where beams and a target correspond to pinning centers and the vortex state domain, respectively. We find a number of trapped fluxes and thus the residual resistance are proportional to the ambient magnetic field and the inverse of the temperature gradient. The obtained formula for the residual resistance is consistent with experimental results. The present model focuses on what happens at the phase transition fronts during a cooling down, reveals why and how the residual resistance depends on the temperature gradient, and naturally explains how the fast cooling works.",1509.03369v1 2020-06-21,A Novel Magnetic Material by Design: Observation of Yb3+ with Spin-1/2 and Possible Superconducting Trace in YbxPt5P,"The localized f-electrons enrich the magnetic properties in rare-earth-based intermetallics. Among those, compounds with heavier 4d and 5d transition metals are even more fascinating because anomalous electronic properties may be induced by the hybridization of 4f and itinerant conduction electrons primarily from the d orbitals. Here, we describe the observation of trivalent Yb3+ with S = 1/2 at low temperatures in YbxPt5P, the first of a new family of materials. YbxPt5P (0.20< x <1) phases were synthesized and structurally characterized. They exhibit a large homogeneity width with the Yb ratio exclusively occupying the 1a site in the anti-CeCoIn5 structure. Moreover, the resistivity measurement of a sample analyzed as Yb0.25Pt5P shows it to exist a complete zero-resistance transition with a critical transition temperature of ~0.6 K, possible superconductivity. However, the zero-resistivity transition was not observed in YbPt5P with antiferromagnetic ordering existing solely. First-principles electronic structure calculations substantiate the antiferromagnetic ground state and indicate that 2D nesting around the Fermi level may give rise to exotic physical properties, such as superconductivity. YbxPt5P appears to be a unique case among materials.",2006.11891v1 2024-03-19,Giant electrode effect on tunneling magnetoresistance and electroresistance in van der Waals intrinsic multiferroic tunnel junctions using VS2,"Van der Waals multiferroic tunnel junctions (vdW-MFTJs) with multiple nonvolatile resistive states are highly suitable for new physics and next-generation storage electronics. However, currently reported vdW-MFTJs are based on two types of materials, i.e., vdW ferromagnetic and ferroelectric materials, forming a multiferroic system. This undoubtedly introduces additional interfaces, increasing the complexity of experimental preparation. Herein, we engineer vdW intrinsic MFTJs utilizing bilayer VS$_2$. By employing the nonequilibrium Green's function combined with density functional theory, we systematically investigate the influence of three types of electrodes (including non-vdW pure metal Ag/Au, vdW metallic 1T-MoS$_2$/2H-PtTe$_2$, and vdW ferromagnetic metallic Fe$_3$GaTe$_2$/Fe$_3$GeTe$_2$) on the electronic transport properties of VS$_2$-based intrinsic MFTJs. We demonstrate that these MFTJs manifest a giant electrode-dependent electronic transport characteristic effect. Comprehensively comparing these electrode pairs, the Fe$_3$GaTe$_2$/Fe$_3$GeTe$_2$ electrode combination exhibits optimal transport properties, the maximum TMR (TER) can reach 10949\% (69\%) and the minimum resistance-area product (RA) is 0.45 $\Omega$$\mu$m$^{2}$, as well as the perfect spin filtering and negative differential resistance effects. More intriguingly, TMR (TER) can be further enhanced to 34000\% (380\%) by applying an external bias voltage (0.1 V), while RA can be reduced to 0.16 $\Omega$$\mu$m$^{2}$ under the influence of biaxial stress (-3\%). Our proposed concept of designing vdW-MFTJs using intrinsic multiferroic materials points towards new avenues in experimental exploration.",2403.12845v2 2001-05-15,Current-Driven Magnetic Memory with Tunable Magnetization Switching,"Co(x nm, x=10nm or 40nm)/Cu(5nm)/Co(2.5nm) layers were deposited between copper electrodes in SiO2 vias. Magnetic states, and the corresponding resistance states, of these devices were switched by electric currents perpendicular to the layers. The I-V loops show asymmetric behavior with hysteresis. When electrons flow in the direction from thick to thin Co layer (positive current), multiple switches were observed on increasing current up to a chosen maximum positive I(write). On decreasing current from I(write), the I-V curve was smooth and characterized by considerably lower resistance. Under reverse current, an abrupt switch to the high resistance state occurred at the current value I(erase)~ -0.9*I(write). Resistance had a maximum at zero current in both states, where the ratio R(high)/R(low) could be as high as factor of four.",0105290v1 2005-12-19,Multiphoton processes in microwave photoresistance of 2D electron system,"We extend our studies of microwave photoresistance of ultra-high mobility two-dimensional electron system (2DES) into the high-intensity, non-linear regime employing both monochromatic and bichromatic radiation. Under high-intensity monochromatic radiation $\omega$ we observe new zero-resistance states (ZRS) which correspond to rational values of $\epsilon=\omega/\omega_C$ ($\omega_C$ is the cyclotron frequency) and can be associated with multiphoton processes. %Formation of these rational ZRS is accompanied by a dramatic reconstruction of the photoresistance spectrum which reveals diminishing, narrowing, and phase reduction of the resistance peaks, as well as overall suppression of resistance at $\epsilon<1/2$. Under bichromatic radiation $\omega_1,\omega_2$ we discover new resistance minimum, possibly a precursor of bichromatic ZRS, which seems to originate from a frequency mixing process, $\omega_1+\omega_2$. These findings indicate that multiphoton processes play important roles in the physics of non-equilibrium transport of microwave-driven 2DES, and suggest new directions for theoretical and experimental studies.",0512479v1 2007-08-17,Developments and the preliminary tests of Resistive GEMs manufactured by a screen printing technology,"We report promising initial results obtained with new resistive-electrode GEM (RETGEM) detectors manufactured, for the first time, using screen printing technology. These new detectors allow one to reach gas gains nearly as high as with ordinary GEM-like detectors with metallic electrodes; however, due to the high resistivity of its electrodes the RETGEM, in contrast to ordinary hole-type detectors, has the advantage of being fully spark protected. We discovered that RETGEMs can operate stably and at high gains in noble gases and in other badly quenched gases, such as mixtures of noble gases with air and in pure air; therefore, a wide range of practical applications, including dosimetry and detection of dangerous gases, is foreseeable. To promote a better understanding of RETGEM technology some comparative studies were completed with metallic-electrode thick GEMs. A primary benefit of these new RETGEMs is that the screen printing technology is easily accessible to many research laboratories. This accessibility encourages the possibility to manufacture these GEM-like detectors with the electrode resistivity easily optimized for particular experimental or practical applications.",0708.2344v1 2016-03-15,Thermo Activated Hysteresis on High Quality Graphene/h-BN Devices,"We report on gate hysteresis in resistance on high quality graphene/h-BN devices. We observe a thermal activated hysteretic behavior in resistance as a function of the applied gate voltage at temperatures above 375K. In order to investigate the origin of the hysteretic phenomenon, we design heterostructures involving graphene/h-BN devices with different underlying substrates such as: SiO2/Si and graphite; where heavily doped silicon and graphite are used as a back gate electrodes, respectively. The gate hysteretic behavior of the resistance shows to be present only in devices with an h-BN/SiO2 interface and is dependent on the orientation of the applied gate electric field and sweep rate. Finally, we suggest a phenomenological model, which captures all of our findings based on charges trapped at the h-BN/SiO2. Certainly, such hysteretic behavior in graphene resistance represents a technological problem for the application of graphene devices at high temperatures, but conversely, it can open new routes for applications on digital electronics and graphene memory devices.",1603.04872v1 2021-09-29,Magnetotransport patterns of collective localization near $ν=1$ in a high-mobility two-dimensional electron gas,"We report complex magnetotransport patterns of the $\nu=1$ integer quantum Hall state in a GaAs/AlGaAs sample from the newest generation with a record high electron mobility. The reentrant integer quantum Hall effect in the flanks of the $\nu=1$ plateau indicates the formation of the integer quantum Hall Wigner solid, a collective insulator. Moreover, at a fixed filling factor, the longitudinal resistance versus temperature in the region of the integer quantum Hall Wigner solid exhibits a sharp peak. Such sharp peaks in the longitudinal resistance versus temperature so far were only detected for bubble phases forming in high Landau levels but were absent in the region of the Anderson insulator. We suggest that in samples of sufficiently low disorder sharp peaks in the longitudinal resistance versus temperature traces are universal transport signatures of all isotropic electron solids that form in the flanks of integer quantum Hall plateaus. We discuss possible origins of these sharp resistance peaks and we draw a stability diagram for the insulating phases in the $\nu$-$T$ phase space.",2109.14649v1 2024-04-29,Mobility and Threshold Voltage Extraction in Transistors with Gate-Voltage-Dependent Contact Resistance,"The mobility of emerging (e.g., two-dimensional, oxide, organic) semiconductors is commonly estimated from transistor current-voltage measurements. However, such devices often experience contact gating, i.e., electric fields from the gate modulate the contact resistance during measurements, which can lead conventional extraction techniques to estimate mobility incorrectly even by a factor >2. This error can be minimized by measuring transistors at high gate-source bias, |$V_\mathrm{gs}$|, but this regime is often inaccessible in emerging devices that suffer from high contact resistance or early gate dielectric breakdown. Here, we propose a method of extracting mobility in transistors with gate-dependent contact resistance that does not require operation at high |$V_\mathrm{gs}$|, enabling accurate mobility extraction even in emerging transistors with strong contact gating. Our approach relies on updating the transfer length method (TLM) and can achieve <10% error even in regimes where conventional techniques overestimate mobility by >2$\times$.",2404.19022v1 2004-09-11,"Magnetic and electron transport properties of the rare-earth cobaltates, La0.7-xLnxCa0.3CoO3 (Ln = Pr, Nd, Gd and Dy) : A case of phase separation","Magnetic and electrical properties of four series of rare earth cobaltates of the formula La0.7-xLnxCa0.3CoO3 with Ln = Pr, Nd, Gd and Dy have been investigated. Compositions close to x = 0.0 contain large ferromagnetic clusters or domains, and show Brillouin-like behaviour of the field-cooled DC magnetization data with fairly high ferromagnetic Tc values, besides low electrical resistivities with near-zero temperature coefficients. The zero-field-cooled data generally show a non-monotonic behaviour with a peak at a temperatures slightly lower than Tc. The near x = 0.0 compositions show a prominent peak corresponding to the Tc in the AC-susceptibility data. The ferromagnetic Tc varies linearly with x or the average radius of the A-site cations, (rA). With increase in x or decrease in (rA), the magnetization value at any given temperature decreases markedly and the AC-susceptibility measurements show a prominent transition arising from small magnetic clusters with some characteristics of a spin-glass. Electrical resistivity increases with increase in x, showed a significant increase around a critical value of x or (rA), at which composition the small clusters also begin to dominate. These properties can be understood in terms of a phase separation scenario wherein large magnetic clusters give way to smaller ones with increase in x, with both types of clusters being present in certain compositions. The changes in magnetic and electrical properties occur parallely since the large ferromagnetic clusters are hole-rich and the small clusters are hole-poor. Variable-range hopping seems to occur at low temperatures in these cobaltates.",0409288v2 2004-11-17,Al substitution in MgB2 crystals: influence on superconducting and structural properties,"Single crystals of Mg1-xAlxB2 have been grown at a pressure of 30 kbar using the cubic anvil technique. Precipitation free crystals with x < 0.1 were obtained as a result of optimization of already developed MgB2 crystal growth procedure. Systematic decrease of the c-axis lattice constant with increasing Al content, when the a-axis lattice constant is practically unchanged, was observed. Variation of the critical temperature on Al content in Mg1-xAlxB2 crystals was found to be slightly different than that one observed for polycrystalline samples since, even a very small substitution of 1-2% of Al leads to the decrease of Tc by about 2-3 K. X-ray and high resolution transmission electron microscopy investigations indicate on the appearance of second precipitation phase in the crystals with x > 0.1. This is in a form of non-superconducting MgAlB4 domains in the structure of superconducting Mg1-xAlxB2 matrix. Resistivity and magnetic investigations show the slight increase of the upper critical field, Hc2, for H//c for the samples with small x, significant reduction of the Hc2 anisotropy at lower temperatures, and decrease of the residual resistance ratio value for Al substituted samples as compared to those of unsubstituted crystals. Superconducting gaps variation as a function of Al content, investigated with point contact spectroscopy for the series of the crystals with Tc in the range from 20 to 37 K, does not indicate on the merging of the gaps with decreasing Tc down to 20 K. It may be related to an appearance of the precipitation phase in the Mg1-xAlxB2 structure.",0411449v2 2007-08-01,Structural and transport properties of GaAs/delta/GaAs/InxGa1-xAs/GaAs quantum wells,"We report results of investigations of structural and transport properties of GaAs/Ga(1-x)In(x)As/GaAs quantum wells (QWs) having a 0.5-1.8 ML thick Mn layer, separated from the QW by a 3 nm thick spacer. The structure has hole mobility of about 2000 cm2/(V*s) being by several orders of magnitude higher than in known ferromagnetic two-dimensional structures. The analysis of the electro-physical properties of these systems is based on detailed study of their structure by means of high-resolution X-ray diffractometry and glancing-incidence reflection, which allow us to restore the depth profiles of structural characteristics of the QWs and thin Mn containing layers. These investigations show absence of Mn atoms inside the QWs. The quality of the structures was also characterized by photoluminescence spectra from the QWs. Transport properties reveal features inherent to ferromagnetic systems: a specific maximum in the temperature dependence of the resistance and the anomalous Hall effect (AHE) observed in samples with both ""metallic"" and activated types of conductivity up to ~100 K. AHE is most pronounced in the temperature range where the resistance maximum is observed, and decreases with decreasing temperature. The results are discussed in terms of interaction of 2D-holes and magnetic Mn ions in presence of large-scale potential fluctuations related to random distribution of Mn atoms. The AHE values are compared with calculations taking into account its ""intrinsic"" mechanism in ferromagnetic systems.",0708.0056v1 2009-08-03,Fabrication of Diamond Nanowires for Quantum Information Processing Applications,"We present a design and a top-down fabrication method for realizing diamond nanowires in both bulk single crystal and polycrystalline diamond. Numerical modeling was used to study coupling between a Nitrogen Vacancy (NV) color center and optical modes of a nanowire, and to find an optimal range of nanowire diameters that allows for large collection efficiency of emitted photons. Inductively coupled plasma (ICP) reactive ion etching (RIE) with oxygen is used to fabricate the nanowires. Drop-casted nanoparticles (including $\mathrm{Au}$, $\mathrm{SiO_{2}}$ and $\mathrm{Al_2O_3}$) as well as electron beam lithography defined spin-on glass and evaporated $\mathrm{Au}$ have been used as an etch mask. We found $\mathrm{Al_2O_3}$ nanoparticles to be the most etch resistant. At the same time FOx e-beam resist (spin-on glass) proved to be a suitable etch mask for fabrication of ordered arrays of diamond nanowires. We were able to obtain nanowires with near vertical sidewalls in both polycrystalline and single crystal diamond. The heights and diameters of the polycrystalline nanowires presented in this paper are $\unit[\approx1]{\mu m}$ and $\unit[120-340]{nm}$, respectively, having a $\unit[200]{nm/min}$ etch rate. In the case of single crystal diamond (types Ib and IIa) nanowires the height and diameter for different diamonds and masks shown in this paper were $\unit[1-2.4]{\mu m}$ and $\unit[120-490]{nm}$ with etch rates between $\unit[190-240]{nm/min}$.",0908.0352v2 2015-08-25,Central Acceptance Testing for Camera Technologies for CTA,"The Cherenkov Telescope Array (CTA) is an international initiative to build the next generation ground based very-high energy gamma-ray observatory. It will consist of telescopes of three different sizes, employing several different technologies for the cameras that detect the Cherenkov light from the observed air showers. In order to ensure the compliance of each camera technology with CTA requirements, CTA will perform central acceptance testing of each camera technology. To assist with this, the Camera Test Facilities (CTF) work package is developing a detailed test program covering the most important performance, stability, and durability requirements, including setting up the necessary equipment. Performance testing will include a wide range of tests like signal amplitude, time resolution, dead-time determination, trigger efficiency, performance testing under temperature and humidity variations and several others. These tests can be performed on fully-integrated cameras using a portable setup at the camera construction sites. In addition, two different setups for performance tests on camera sub-units are being built, which can provide early feedback for camera development. Stability and durability tests will include the long-term functionality of movable parts, water tightness of the camera housing, temperature and humidity cycling, resistance to vibrations during transport or due to possible earthquakes, UV-resistance of materials and several others. Some durability tests will need to be contracted out because they will need dedicated equipment not currently available within CTA. The planned test procedures and the current status of the test facilities will be presented.",1508.06074v1 2016-08-28,Magnetic order and spin-orbit coupled Mott state in double perovskite (La$_{1-x}$Sr$_x$)$_2$CuIrO$_6$,"Double-perovskite oxides that contain both 3d and 5d transition metal elements have attracted growing interest as they provide a model system to study the interplay of strong electron interaction and large spin-orbit coupling (SOC). Here, we report on experimental and theoretical studies of the magnetic and electronic properties of double-perovskites (La$_{1-x}$Sr$_x$)$_2$CuIrO$_6$ ($x$ = 0.0, 0.1, 0.2, and 0.3). The undoped La$_2$CuIrO$_6$ undergoes a magnetic phase transition from paramagnetism to antiferromagnetism at T$_N$ $\sim$ 74 K and exhibits a weak ferromagnetic behavior below $T_C$ $\sim$ 52 K. Two-dimensional magnetism that was observed in many other Cu-based double-perovskites is absent in our samples, which may be due to the existence of weak Cu-Ir exchange interaction. First-principle density-functional theory (DFT) calculations show canted antiferromagnetic (AFM) order in both Cu$^{2+}$ and Ir$^{4+}$ sublattices, which gives rise to weak ferromagnetism. Electronic structure calculations suggest that La$_2$CuIrO$_6$ is an SOC-driven Mott insulator with an energy gap of $\sim$ 0.3 eV. Sr-doping decreases the magnetic ordering temperatures ($T_N$ and $T_C$) and suppresses the electrical resistivity. The high temperatures resistivity can be fitted using a variable-range-hopping model, consistent with the existence of disorders in these double-pervoskite compounds.",1608.07763v2 2017-10-11,Fermi surface with Dirac fermions in CaFeAsF determined via quantum oscillation measurements,"Despite the fact that 1111-type iron arsenides hold the record transition temperature of iron-based superconductors, their electronic structures have not been studied much because of the lack of high-quality single crystals. In this study, we completely determine the Fermi surface in the antiferromagnetic state of CaFeAsF, a 1111 iron-arsenide parent compound, by performing quantum oscillation measurements and band-structure calculations. The determined Fermi surface consists of a symmetry-related pair of Dirac electron cylinders and a normal hole cylinder. From analyses of quantum-oscillation phases, we demonstrate that the electron cylinders carry a nontrivial Berry phase $\pi$. The carrier density is of the order of 10$^{-3}$ per Fe. This unusual metallic state with the extremely small carrier density is a consequence of the previously discussed topological feature of the band structure which prevents the antiferromagnetic gap from being a full gap. We also report a nearly linear-in-$B$ magnetoresistance and an anomalous resistivity increase above about 30 T for $B \parallel c$, the latter of which is likely related to the quantum limit of the electron orbit. Intriguingly, the electrical resistivity exhibits a nonmetallic temperature dependence in the paramagnetic tetragonal phase ($T >$ 118 K), which may suggest an incoherent state. Our study provides a detailed knowledge of the Fermi surface in the antiferromagnetic state of 1111 parent compounds and moreover opens up a new possibility to explore Dirac-fermion physics in those compounds.",1710.03938v3 2020-04-23,Ultralow Schottky Barriers in hBN-Encapsulated Monolayer WSe$_2$ Tunnel Field-Effect Transistors,"To explore the potential of field-effect transistors (FETs) based on monolayers of the two-dimensional semiconducting channel(SC) for spintronics, the two most important issues are to ensure the formation of variable low resistive tunnel ferromagnetic contacts(FC), and to preserve intrinsic properties of the SC during fabrication. Large Schottky barriers lead to the formation of high resistive contacts and methods adopted to control the barriers often alter the intrinsic properties of the SC. This work aims at addressing both issues in fully encapsulated monolayer WSe$_2$ FETs by using bi-layer h-BN as a tunnel barrier at the FC/SC interface. We investigate the electrical transport in monolayer WSe$_2$ FETs with current-in-plane geometry that yields hole mobilities $\sim$ 38.3 $cm^{2}V^{-1}s^{-1}$ at 240 K and On/Off ratios of the order of 10$^7$, limited by the contact regions. We have achieved ultralow effective Schottky barrier ($\sim$ 5.34 meV) with encapsulated tunneling device as opposed to a non-encapsulated device in which the barrier heights are considerably higher. These observations provide an insight into the electrical behavior of the FC/h-BN/SC/h-BN heterostructures and such control over the barrier heights opens up the possibilities for WSe$_2$-based spintronic devices.",2004.10962v1 2015-04-23,Fowler-Nordheim Plot Analysis: a Progress Report,"The commonest method of characterizing a cold field electron emitter is to measure its current-voltage characteristics, and the commonest method of analysing these characteristics is by means of a Fowler-Nordheim (FN) plot. This tutorial/review-type paper outlines a more systematic method of setting out the Fowler-Nordheim-type theory of cold field electron emission, and brings together and summarises the current state of work by the authors on developing the theory and methodology of FN plot analysis. This has turned out to be far more complicated than originally expected. Emphasis is placed in this paper on: (a) the interpretation of FN-plot slopes, which is currently both easier and of more experimental interest than the analysis of FN-plot intercepts; and (b) preliminary explorations into developing methodology for interpreting current-voltage characteristics when there is series resistance in the conduction path from the high-voltage generator to the emitter's emitting regions. This work reinforces our view that FN-plot analysis is best carried out on the raw measured current-voltage data, without pre-conversion into another data format, particularly if series resistance is present in the measuring circuit. Relevant formulae are given for extracting field-enhancement-factor values from such an analysis.",1504.06134v7 2018-07-07,Three-dimensional quantum Hall effect and metal-insulator transition in ZrTe5,"Symmetry, dimensionality, and interaction are crucial ingredients for phase transitions and quantum states of matter. As a prominent example, the integer quantum Hall effect (QHE) represents a topological phase generally regarded as characteristic for two-dimensional (2D) electronic systems, and its many aspects can be understood without invoking electron-electron interaction. The intriguing possibility of generalizing QHE to three-dimensional (3D) systems was proposed decades ago, yet it remains elusive experimentally. Here, we report clear experimental evidence for the 3D QHE observed in bulk ZrTe5 crystals. Owing to the extremely high sample quality, the extreme quantum limit with only the lowest Landau level occupied can be achieved by an applied magnetic field as low as 1.5 T. Remarkably, in this regime, we observe a dissipationless longitudinal resistivity rho_xx=0 accompanied with a well-developed Hall resistivity plateau rho_xy=(1\pm0.1) h/e^2 (\lambda_(F,z)/2), where \lambda_(F,z) is the Fermi wavelength along the field direction (z axis). This striking result strongly suggests a Fermi surface instability driven by the enhanced interaction effects in the extreme quantum limit. In addition, with further increasing magnetic field, both rho_xx and rho_xy increase dramatically and display an interesting metal-insulator transition, representing another magnetic field driven quantum phase transition. Our findings not only unambiguously reveal a novel quantum state of matter resulting from an intricate interplay among dimensionality, interaction, and symmetry breaking, but also provide a promising platform for further exploration of more exotic quantum phases and transitions in 3D systems.",1807.02678v2 2019-01-14,Detailed physical property characterization of FeTe1-xSex x = 0.0 to 0.50 single crystals,"Here, we report self flux single crystal growth of FeTe1-xSex for x = 0 to 0.50 series via solid state reaction route,the resulted crystals as seen are shiny. X Ray diffraction performed on the surface of crystals elucidated the growth in 00l plane, i.e. orientation in c direction only. Scanning electron microscopy (SEM) images showed slab like morphology and EDX (Energy dispersive X ray analyzer) confirmed that the crystals are closed to their designed compositions. Rietveld analysis of the XRD patterns of crushed crystal powders showed that the cell parameters decrease with Se content increase. Coupled magnetic and structural phase transition temperature, seen as a step in resistivity for the lower Se concentration and it is not detected for higher x values. Superconductivity is observed by resistivity measurement for higher Se concentration with a maximum temperature of 14K at x = 0.50. Thermally Activated Flux Flow (TAFF) analysis based on high field transport measurements in superconducting region done for x = 0.20 crystal. Raman spectroscopy at room temperature of synthesized samples exhibits all the allowed phonon modes with slight shift to higher frequency with Se content. Mossbauer spectra of FeTe1-xSex crystals series were recorded at 300 and 5K. At 5K, the average hyperfine field decreases systematically with Se content increase from 10.6 to 6.1Tesla for x = 0.0 to x = 0.20 samples. This indicates a possibility of co-existing magnetism and superconductivity in x = 0.07 to 0.20 crystals. For x = 0.50 sample, no hyperfine field related to magnetic ordering is seen. Based on above results, detailed phase diagram of the FeTe1-xSex compounds is defined in the present study.",1901.04224v1 2019-01-24,Fascinating interplay between Charge Density Wave Order and magnetic field in Non-magnetic Rare-Earth Tritelluride LaTe$_{3}$,"Charge density wave (CDW) states in solids bear an intimate connection to underlying fermiology. Modification of the latter by a suitable perturbation provides an attractive handle to unearth novel CDW states. Here, we combine extensive magnetotransport experiments and first-principles electronic structure calculations on a non-magnetic tritelluride LaTe$_{3}$ single crystal to uncover phenomena rare in CDW systems: $(i)$ hump-like feature in the temperature dependence of resistivity at low temperature under application of magnetic field, which moves to higher temperature with increasing field strength, $(ii)$ highly anisotropic large transverse magnetoresistance (MR) upon rotation of magnetic field about current parallel to crystallographic c-axis, (iii) anomalously large positive MR with spike-like peaks at characteristic angles when the angle between current and field is varied in the bc-plane, (iv) extreme sensitivity of the angular variation of MR on field and temperature. Moreover, our Hall measurement reveals remarkably high carrier mobility $\sim$ 33000 cm$^{2}$/Vs, which is comparable to that observed in some topological semimetals. These novel observations find a comprehensive explication in our density functional theory (DFT) and dynamical mean field theory (DMFT) calculations that capture field-induced electronic structure modification in LaTe$_{3}$. The band structure theory together with transport calculations suggest the possibility of a second field-induced CDW transition from the field-reconstructed Fermi surface, which qualitatively explains the hump in temperature dependence of resistivity at low temperature. Thus, our study exposes the novel manifestations of the interplay between CDW order and field-induced electronic structure modifications in LaTe$_{3}$, and establishes a new route to tune CDW states by perturbations like magnetic field.",1901.08267v2 2019-06-09,Spin dynamics and unconventional magnetism in insulating La$_{(1-2x)}$Sr$_{2x}$Co$_{(1-x)}$Nb$_{x}$O$_3$,"We study the structural, magnetic, transport and electronic properties of LaCoO$_3$ with Sr/Nb co-substitution, i.e., La$_{(1-2x)}$Sr$_{2x}$Co$_{(1-x)}$Nb$_{x}$O$_3$ using x-ray and neutron diffraction, dc and ac-magnetization, neutron depolarization, dc-resistivity and photoemission measurements. The powder x-ray and neutron diffraction data were fitted well with the rhombohedral crystal symmetry (space group \textit{R$\bar{3}$c}) in Rietveld refinement analysis. The calculated effective magnetic moment ($\approx$3.85~$\mu_B$) and average spin ($\approx$1.5) of Co ions from the analysis of magnetic susceptibility data are consistent with 3+ state of Co ions in intermediate-spin (IS) and high-spin (HS) states in the ratio of $\approx$50:50, i.e., spin-state of Co$^{3+}$ is preserved at least up to $x=$ 0.1 sample. Interestingly, the magnetization values were significantly increased with respect to the $x=$ 0 sample, and the M-H curves show non-saturated behavior up to an applied maximum magnetic field of $\pm$70 kOe. The ac-susceptibility data show a shift in the freezing temperature with excitation frequency and the detailed analysis confirm the slower dynamics and a non-zero value of the Vogel-Fulcher temperature T$_0$, which suggests for the cluster spin glass. The unusual magnetic behavior indicates the presence of complex magnetic interactions at low temperatures. The dc-resistivity measurements show the insulating nature in all the samples. However, relatively large density of states $\approx$10$^{22}$ eV$^{-1}$cm$^{-3}$ and low activation energy $\approx$130~meV are found in $x=$ 0.05 sample. Using x-ray photoemission spectroscopy, we study the core-level spectra of La 3$d$, Co 2$p$, Sr 3$d$, and Nb 3$d$ to confirm the valence state.",1906.03659v1 2019-10-14,First predictive simulations for deuterium shattered pellet injection in ASDEX Upgrade,"First simulations of deuterium shattered pellet injection (SPI) into an ASDEX Upgrade H-Mode plasma with the JOREK MHD code are presented. Resistivity is increased by one order of magnitude in most simulations to reduce computational costs and allow for extensive parameter scans. The effect of various physical parameters onto MHD activity and thermal quench (TQ) dynamics is studied and the influence of MHD onto ablation is shown. TQs are obtained quickly after injection in most simulations with a typical duration of 100 microseconds, which slows down at lower resistivity. Although the n=1 magnetic perturbation dominates in the simulations, toroidal harmonics up to n=10 contribute to stochastization and stochastic transport in the plasma core. The post-TQ density profile remains hollow for a few hundred microseconds. However, when flux surfaces re-form around the magnetic axis, the density has become monotonic again suggesting a beneficial behaviour for runaway electron avoidance/mitigation. With $10^{21}$ atoms injected, the TQ is typically incomplete and triggered when the shards reach the q=2 rational surface. At a larger number of injected atoms, the TQ can set in even before the shards reach this surface. For low field side injection considered here, repeated formation of outward convection cells is observed in the ablation region reducing material assimilation. Responsible is a sudden rise of pressure in the high density cloud when the stochastic region expands further releasing heat from the hot core. After the TQ, strong sheared poloidal rotation is created by Maxwell stress, which contributes to re-formation of flux surfaces.",1910.06095v4 2020-08-25,Isospin Pomeranchuk effect and the entropy of collective excitations in twisted bilayer graphene,"In condensed matter systems, higher temperatures typically disfavors ordered phases leading to an upper critical temperature for magnetism, superconductivity, and other phenomena. A notable exception is the Pomeranchuk effect in 3He, in which the liquid ground state freezes upon increasing the temperature due to the large entropy of the paramagnetic solid phase. Here we show that a similar mechanism describes the finite temperature dynamics of spin and valley-isospins in magic-angle twisted bilayer graphene. Most strikingly a resistivity peak appears at high temperatures near superlattice filling factor nu = -1, despite no signs of a commensurate correlated phase appearing in the low-temperature limit. Tilted field magnetotransport and thermodynamic measurements of the inplane magnetic moment show that the resistivity peak is adiabatically connected to a finite-field magnetic phase transition at which the system develops finite isospin polarization. These data are suggestive of a Pomeranchuk-type mechanism, in which the entropy of disordered isospin moments in the ferromagnetic phase stabilizes it relative to an isospin unpolarized Fermi liquid phase at elevated temperatures. Measurements of the entropy, S/kB indeed find it to be of order unity per unit cell area, with a measurable fraction that is suppressed by an in-plane magnetic field consistent with a contribution from disordered physical spins. In contrast to 3He, however, no discontinuities are observed in the thermodynamic quantities across this transition. Our findings imply a small isospin stiffness, with implications for the nature of finite temperature transport as well as the mechanisms underlying isospin ordering and superconductivity in twisted bilayer graphene and related systems.",2008.10830v4 2021-05-18,One-reactor vacuum and plasma synthesis of transparent conducting oxide nanotubes and nanotrees: from single wire conductivity to ultra-broadband perfect absorbers in the NIR,"The eventual exploitation of one-dimensional nanomaterials yet needs the development of scalable, high yield, homogeneous, and environmentally friendly methods able to meet the requirements for the fabrication of under design functional nanomaterials. In this article, we demonstrate a vacuum and plasma one-reactor approach for the synthesis of the fundamental common element in solar energy and optoelectronics, i.e. the transparent conducting electrode but in the form of nanotubes and nanotrees architectures. Although the process is generic and can be used for a variety of TCOs and wide-bandgap semiconductors, we focus herein on Indium Doped Tin Oxide (ITO) as the most extended in the previous applications. This protocol combines widely applied deposition techniques such as thermal evaporation for the formation of organic nanowires serving as 1D and 3D soft templates, deposition of polycrystalline layers by magnetron sputtering, and removal of the template by simply annealing under mild vacuum conditions. The process variables are tuned to control the stoichiometry, morphology, and alignment of the ITO nanotubes and nanotrees. Four-probe characterization reveals the improved lateral connectivity of the ITO nanotrees and applied on individual nanotubes shows resistivities as low as 3.5 +/- 0.9 x 10-4 {\Omega}.cm, a value comparable to single-crystalline counterparts. The assessment of diffuse reflectance and transmittance in the UV-VIS range confirms the viability of the supported ITO nanotubes as a random optical media working as strong scattering layers. Further ability to form ITO nanotrees opens the path for practical applications as ultra-broadband absorbers in the NIR. The demonstrated low resistivity and optical properties of these ITO nanostructures open the way for their use in LEDs, IR shield, energy harvesting, nanosensors, and photoelectrochemical applications",2105.08751v1 2021-09-01,Interaction driven giant thermopower in magic-angle twisted bilayer graphene,"Magic-angle twisted bilayer graphene (MtBLG) has proven to be an extremely promising new platform to realize and study a host of emergent quantum phases arising from the strong correlations in its narrow bandwidth flat band. In this regard, thermal transport phenomena like thermopower, in addition to being coveted technologically, is also sensitive to the particle-hole (PH) asymmetry, making it a crucial tool to probe the underlying electronic structure of this material. We have carried out thermopower measurements of MtBLG as a function of carrier density, temperature and magnetic field, and report the observation of an unusually large thermopower reaching up to a value as high as $\sim \bf{100\mu V/K}$ at a low temperature of 1K. Surprisingly, our observed thermopower exhibiting peak-like features in close correspondence to the resistance peaks around the integer Moire fillings, including the Dirac Point, violating the Mott formula. %Surprisingly, our observed thermopower exhibits peak-like features in close correspondence to the resistance peaks around the integer Moire fillings, including the Dirac Point, which completely violates the Mott formula. We show that the large thermopower peaks and their %non-monotonic dependence with temperature and magnetic field associated behaviour arise from the emergent highly PH asymmetric electronic structure due to the cascade of Dirac revivals. Furthermore, the thermopower shows an anomalous peak around the superconducting transition on the hole side and points towards the possible role of enhanced superconducting fluctuations in MtBLG.",2109.00361v2 2022-06-13,Long-range magnetic order in the anisotropic triangular lattice system CeCd3As3,"We report the physical properties of $R$Cd$_{3}$As$_{3}$ ($R$ = La and Ce) compounds, crystallized into a hexagonal ScAl$_{3}$C$_{3}$-type structure ($P$6$_{3}$/mmc) such that the $R$ sublattice forms a spin-orbit coupled triangular lattice. Magnetic susceptibility measurements indicate the 4$f$ electrons of Ce$^{3+}$ ions are well localized and reveal a large magnetic anisotropy. The electrical resistivity and specific heat measurement for $R$Cd$_{3}$As$_{3}$ exhibit an anomaly at high temperatures ($T_{0}$ $\sim$ 63 K for $R$ = La and $T_{0}$ $\sim$ 136 K for $R$ = Ce), most likely due to a structural transition. Specific heat measurements for CeCd$_{3}$As$_{3}$ clearly indicate a long range magnetic order below $T_{N}$ = 0.42 K. Although the magnetic contribution to the specific heat $C_{m}/T$ increases significantly below $\sim$ 10 K, the electrical resistivity for CeCd$_{3}$As$_{3}$ follows typical, metallic behavior inconsistent with Kondo lattice systems. In CeCd$_3$As$_3$ only $\sim$ 40 $\%$ of the $R \ln(2)$ magnetic entropy is recovered by $T_N$ and the $R$ln(2) entropy is fully achieved at about the Curie-Weiss temperature $|\theta_{p}|$. Unusually, based on our current investigations, the magnetic specific heat below $|\theta_{p}|$ is not attributed to a Kondo contribution, but rather associated with the magnetic ordering and frustration on the triangular lattice. Specific heat measurements in applied magnetic field show a negligible variation of $T_{N}$ for $H \parallel c$, whereas a suppression of $T_{N}$ is observed above 40 kOe for $H \parallel ab$. Such behavior is consistent with the application a magnetic field within the $ab$-plane breaking the triangular symmetry and partially relieving the magnetic frustration in this system.",2206.06403v1 2022-11-05,"Effect of various electron and hole transport layers on the performance of CsPbI3-based perovskite solar cells: A numerical investigation in DFT, SCAPS-1D, and wxAMPS frameworks","CsPbI3 has recently received tremendous attention as a possible absorber of perovskite solar cells (PSCs). However, CsPbI3-based PSCs have yet to achieve the high performance of the hybrid PSCs. In this work, we performed a density functional theory (DFT) study using the Cambridge Serial Total Energy Package (CASTEP) code for the cubic CsPbI3 absorber to compare and evaluate its structural, electronic, and optical properties. The calculated electronic band gap (Eg) using the GGA-PBE approach of CASTEP was 1.483 eV for this CsPbI3 absorber. Moreover, the computed density of states (DOS) exhibited the dominant contribution from the Pb-5d orbital, and most charge also accumulated for the Pb atom as seen from the electronic charge density map. Fermi surface calculation showed multiband character, and optical properties were computed to investigate the optical response of CsPbI3. Furthermore, we used IGZO, SnO2, WS2, CeO2, PCBM, TiO2, ZnO, and C60 as the electron transport layers (ETLs), and Cu2O, CuSCN, CuSbS2, Spiro-MeOTAD, V2O5, CBTS, CFTS, P3HT, PEDOT: PSS, NiO, CuO, and CuI as the hole transport layers (HTLs) to identify the best HTL/CsPbI3/ETL combinations using the SCAPS-1D solar cell simulation software. Among 96 device structures, the best-optimized device structure, ITO/TiO2/CsPbI3/CBTS/Au was identified, which exhibited an efficiency of 17.9%. The effect of absorber and ETL thickness, series resistance, shunt resistance, and operating temperature was also evaluated for the six best devices along with their corresponding generation rate, recombination rate, capacitance-voltage, current density-voltage, and quantum efficiency characteristics. The obtained results from SCAPS-1D were also compared with wxAMPS simulation software.",2211.02968v1 2023-01-30,Infrared ellipsometry study of the charge dynamics in K3p-terphenyl,"We report an infrared ellipsometry study of the charge carrier dynamics in polycrystalline Kxp-terphenyl samples with nominal $x=3$, for which signatures of high-temperature superconductivity were previously reported. The infrared spectra are dominated by two Lorentzian bands with maxima around 4 000 cm$^{-1}$ and 12 000 cm$^{-1}$ which, from a comparison with calculations based on a H\""uckel model are assigned to intra-molecular excitations of $\pi$ electrons of the anionic p-terphenyl molecules. The inter-molecular electronic excitations are much weaker and give rise to a Drude peak and a similarly weak Lorentzian band around 220 cm$^{-1}$. A dc resistivity of about 0.3 $\Omega$ cm at 300 K is deduced from the IR data, comparable to values measured by electrical resistivity on a twin sample. The analysis of the temperature dependence of the low-frequency response reveals a gradual decrease of the plasma frequency and the scattering rate of the Drude peak below 300 K that gets anomalously enhanced below 90 K. The corresponding missing spectral weight of the Drude peak appears blue-shifted towards the Lorentz-band at 220 cm$^{-1}$. This characteristic blue-shift signifies an enhanced localization of the charge carriers at low temperatures and contrasts the behavior expected for a bulk superconducting state for which the missing spectral weight would be redshifted to a delta-function at zero frequency that accounts for the loss-free response of the superconducting condensate. Our data might still be compatible with a filamentary superconducting state with a volume fraction well below the percolation limit for which the spatial confinement of the condensate can result in a plasmonic resonance at finite frequency.",2302.10097v2 2023-08-04,Observation of Fractionally Quantized Anomalous Hall Effect,"The integer quantum anomalous Hall (QAH) effect is a lattice analog of the quantum Hall effect at zero magnetic field. This striking transport phenomenon occurs in electronic systems with topologically nontrivial bands and spontaneous time-reversal symmetry breaking. Discovery of its putative fractional counterpart in the presence of strong electron correlations, i.e., the fractional quantum anomalous Hall (FQAH) effect, would open a new chapter in condensed matter physics. Here, we report the direct observation of both integer and fractional QAH effects in electrical measurements on twisted bilayer MoTe$_2$. At zero magnetic field, near filling factor $\nu = -1$ (one hole per moir\'e unit cell) we see an extended integer QAH plateau in the Hall resistance $R_\text{xy}$ that is quantized to $h/e^2 \pm 0.1 \%$ while the longitudinal resistance $R_\text{xx}$ vanishes. Remarkably, at $\nu=-2/3$ and $-3/5$ we see plateau features in $R_\text{xy}$ at $3h/2e^2 \pm 1\%$ and $5h/3e^2 \pm 3\%$, respectively, while $R_\text{xx}$ remains small. All these features shift linearly in an applied magnetic field with slopes matching the corresponding Chern numbers $-1$, $-2/3$, and $-3/5$, precisely as expected for integer and fractional QAH states. In addition, at zero magnetic field, $R_\text{xy}$ is approximately $2h/e^2$ near half filling ($\nu = -1/2$) and varies linearly as $\nu$ is tuned. This behavior resembles that of the composite Fermi liquid in the half-filled lowest Landau level of a two-dimensional electron gas at high magnetic field. Direct observation of the FQAH and associated effects paves the way for researching charge fractionalization and anyonic statistics at zero magnetic field.",2308.02657v1 2023-09-29,Fractional Quantum Anomalous Hall Effect in a Graphene Moire Superlattice,"The fractional quantum anomalous Hall effect (FQAHE), the analog of the fractional quantum Hall effect1 at zero magnetic field, is predicted to exist in topological flat bands under spontaneous time-reversal-symmetry breaking. The demonstration of FQAHE could lead to non-Abelian anyons which form the basis of topological quantum computation. So far, FQAHE has been observed only in twisted MoTe2 (t-MoTe2) at moire filling factor v > 1/2. Graphene-based moire superlattices are believed to host FQAHE with the potential advantage of superior material quality and higher electron mobility. Here we report the observation of integer and fractional QAH effects in a rhombohedral pentalayer graphene/hBN moire superlattice. At zero magnetic field, we observed plateaus of quantized Hall resistance Rxy = h/(ve^2) at filling factors v = 1, 2/3, 3/5, 4/7, 4/9, 3/7 and 2/5 of the moire superlattice respectively. These features are accompanied by clear dips in the longitudinal resistance Rxx. In addition, at zero magnetic field, Rxy equals 2h/e^2 at v = 1/2 and varies linearly with the filling factor-similar to the composite Fermi liquid (CFL) in the half-filled lowest Landau level at high magnetic fields. By tuning the gate displacement field D and v, we observed phase transitions from CFL and FQAH states to other correlated electron states. Our graphene system provides an ideal platform for exploring charge fractionalization and (non-Abelian) anyonic braiding at zero magnetic field, especially considering a lateral junction between FQAHE and superconducting regions in the same device.",2309.17436v4 2024-03-20,Effect of annealing on the hot salt corrosion resistance of the fine-grained titanium alpha-alloy Ti-2.5Al-2.6Zr obtained via cold Rotary Swaging,"A hot salt corrosion (HSC) test was performed on the fine-grained titanium alpha-alloy Ti-2.5Al-2.6Zr (Russian industrial alloy PT-7M). The ultrafine-grained (UFG) microstructure in the titanium alpha-alloy was formed via cold Rotary Swaging. The grain size and volume fraction of the recrystallized microstructure in the alloy were varied by choosing appropriate annealing temperatures and times. The microstructure and corrosion resistance of UFG alloys were studied after 30 min of annealing at 500-700C and after 1000 h of annealing at 250C. Metallographic studies were carried out to investigate the effects of annealing on the nature and extent of corrosive damage in the titanium alpha-alloy Ti-2.5Al-2.6Zr. After HSC tests, surface analyses of the titanium alpha-alloy samples were conducted using X-ray diffraction and electron microscopy. During the HSC testing of the titanium alpha-alloy Ti-2.5Al-2.6Zr, a competitive interaction between intergranular corrosion (IGC) and pitting corrosion was observed. To the best of our knowledge, it was shown for the first time that annealing affects the relationship among the IGC, pitting corrosion and uniform corrosion rates of the titanium alloy. Prolonged low-temperature annealing at 250C resulted in a more pronounced increase in the uniform corrosion rate than short-term high-temperature annealing for 30 min at 500-700C. An in-depth analysis of the effect of the structure and phase composition of the grain boundaries on the susceptibility of the alpha-alloy Ti-2.5Al-2.6Zr to HSC was conducted.",2403.13587v1 2024-04-23,Magnetic anisotropy in single-crystalline antiferromagnetic Mn$_2$Au,"Multiple recent studies have identified the metallic antiferromagnet Mn$_2$Au to be a candidate for spintronic applications due to apparent in-plane anisotropy, preserved magnetic properties above room temperature, and current-induced N\'eel vector switching. Crystal growth is complicated by the fact that Mn$_2$Au melts incongruently. We present a bismuth flux method to grow millimeter-scale bulk single crystals of Mn$_2$Au in order to examine the intrinsic anisotropic electrical and magnetic properties. Flux quenching experiments reveal that the Mn$_2$Au crystals precipitate below 550{\deg}C, about 100{\deg}C below the decomposition temperature of Mn$_2$Au. Bulk Mn$_2$Au crystals have a room-temperature resistivity of 16-19 $\mu\Omega$-cm and a residual resistivity ratio of 41. Mn$_2$Au crystals have a dimensionless susceptibility on the order of 10$^{-4}$, comparable to calculated and experimental reports on powder samples. Single-crystal neutron diffraction confirms the in-plane magnetic structure. The tetragonal symmetry of Mn$_2$Au constrains the $ab$-plane magnetic susceptibility to be constant, meaning that $\chi_{100}=\chi_{110}$ in the low-field limit, below any spin-flop transition. We find that three measured magnetic susceptibilities $\chi_{100}$, $\chi_{110}$, and $\chi_{001}$ are the same order of magnitude and agree with the calculated prediction, meaning the low-field susceptibility of Mn$_2$Au is quite isotropic, despite clear differences in $ab$-plane and $ac$-plane magnetocrystalline anisotropy. Mn$_2$Au is calculated to have an extremely high in-plane spin-flop field above 30 T, which is much larger than that of another in-plane antiferromagnet Fe$_2$As (less than 1 T). The subtle anisotropy of intrinsic susceptibilities may lead to dominating effects from shape, crystalline texture, strain, and defects in devices that attempt spin readout in Mn$_2$Au.",2404.15525v1 2006-05-06,Three-dimensionality of field-induced magnetism in a high-temperature superconductor,"Many physical properties of high-temperature (high-Tc) superconductors are two-dimensional phenomena derived from their square planar CuO2 building blocks. This is especially true of the magnetism from the copper ions. As mobile charge carriers enter the CuO2 layers, the antiferromagnetism of the parent insulators, where each copper spin is antiparallel to its nearest neighbours1, evolves into a fluctuating state where the spins show tendencies towards magnetic order of a longer periodicity. For certain charge carrier densities, quantum fluctuations are sufficiently suppressed to yield static long-period order2,3,4,5,6, and external magnetic fields also induce such order7,8,9,10,11,12. Here we show that in contrast to the chemically-controlled order in superconducting samples, the field-induced order in these same samples is actually three-dimensional, implying significant magnetic linkage between the CuO2 planes. The results are important because they show that there are three-dimensional magnetic couplings which survive into the superconducting state, and coexist with the crucial inter-layer couplings responsible for three-dimensional superconductivity. Both types of coupling will straighten the vortex lines, implying that we have finally established a direct link between technical superconductivity, which requires zero electrical resistance in an applied magnetic field and depends on vortex dynamics, and the underlying antiferromagnetism of the cuprates.",0605164v1 2008-06-24,Crystal structure and phase transitions across the metal-superconductor boundary in the SmFeAsO1-xFx (0 < x < 0.20) family,"The fluorine-doped rare-earth iron oxyarsenides, REFeAsO1-xFx (RE =rare earth) have recently emerged as a new family of high-temperature superconductors with transition temperatures (Tc) as high as 55 K (refs 1-4). Early work has provided compelling evidence that the undoped parent materials exhibit spin-density-wave (SDW) antiferromagnetic order and undergo a structural phase transition from tetragonal to orthorhombic crystal symmetry upon cooling.5 Both the magnetic and structural instabilities are suppressed upon doping with fluoride ions before the appearance of superconductivity.6,7 Here we use high-resolution synchrotron X-ray diffraction to study the structural properties of SmFeAsO1-xFx (0 < x < 0.20) in which superconductivity emerges near x ~ 0.07 and Tc increases monotonically with doping up to x ~ 0.20.8 We find that orthorhombic symmetry survives through the metal-superconductor boundary well into the superconducting regime 2 and the structural distortion is only suppressed at doping levels, x > 0.15 when the superconducting phase becomes metrically tetragonal. Remarkably this crystal symmetry crossover coincides with reported drastic anomalies in the resistivity and the Hall coefficient8 and a switch of the pressure coefficient of Tc from positive to negative,9 thereby implying that the low-temperature structure plays a key role in defining the electronic properties of these superconductors.",0806.3962v1 2012-04-23,Integrating Functional Oxides with Graphene,"Graphene-oxide hybrid structures offer the opportunity to combine the versatile functionalities of oxides with the excellent electronic transport in graphene. Understanding and controlling how the dielectric environment affects the intrinsic properties of graphene is also critical to fundamental studies and technological development of graphene. Here we review our recent effort on understanding the transport properties of graphene interfaced with ferroelectric Pb(Zr,Ti)O_3 (PZT) and high-k HfO_2. Graphene field effect devices prepared on high-quality single crystal PZT substrates exhibit up to tenfold increases in mobility compared to SiO_2-gated devices. An unusual and robust resistance hysteresis is observed in these samples, which is attributed to the complex surface chemistry of the ferroelectric. Surface polar optical phonons of oxides in graphene transistors play an important role in the device performance. We review their effects on mobility and the high source-drain bias saturation current of graphene, which are crucial for developing graphene-based room temperature high-speed amplifiers. Oxides also introduce scattering sources that limit the low temperature electron mobility in graphene. We present a comprehensive study of the transport and quantum scattering times to differentiate various scattering scenarios and quantitatively evaluate the density and distribution of charged impurities and the effect of dielectric screening. Our results can facilitate the design of multifunctional nano-devices utilizing graphene-oxide hybrid structures.",1204.5161v1 2012-08-30,"High-pressure flux growth, structural, and superconducting properties of LnFeAsO (Ln = Pr, Nd, Sm) single crystals","Single crystals of the LnFeAsO (Ln1111, Ln = Pr, Nd, and Sm) family with lateral dimensions up to 1 mm were grown from NaAs and KAs flux at high pressure. The crystals are of good structural quality and become superconducting when O is partially substituted by F (PrFeAsO1-xFx and NdFeAsO1-xFx) or when Fe is substituted by Co (SmFe1-xCoxAsO). From magnetization measurements, we estimate the temperature dependence and anisotropy of the upper critical field and the critical current density of underdoped PrFeAsO0.7F0.3 crystal with Tc = 25 K. Single crystals of SmFe1-xCoxAsO with maximal Tc up to 16.3 K for x = 0.08 were grown for the first time. From transport and magnetic measurements we estimate the critical fields and their anisotropy, and find these superconducting properties to be quite comparable to the ones in SmFeAsO1-xFx with a much higher Tc of = 50 K. The magnetically measured critical current densities are as high as 109 A/m2 at 2 K up to 7 T, with indication of the usual fishtail effect. The upper critical field estimated from resistivity measurements is anisotropic with slopes of -8.7 T/K (H // ab-plane) and -1.7 T/K (H // c-axis). This anisotropy (= 5) is similar to that in other Ln1111 crystals with various higher Tc s.",1208.6207v2 2013-09-06,MgB2 nonlinear properties investigated under localized high rf magnetic field excitation-report 2,"The high transition temperature and low surface resistance of MgB2 attracts interest in its potential application in superconducting radio frequency accelerating cavities. However, compared to traditional Nb cavities, the viability of MgB2 at high rf fields is still open to question. Our approach is to study the nonlinear electrodynamics of the material under localized rf magnetic fields. Because of the presence of the small superconducting gap in the $\pi$ band, the nonlinear response of MgB2 at low temperature is potentially complicated compared to a single-gap s-wave superconductor such as Nb. Understanding the mechanisms of nonlinearity coming from the two-band structure of MgB2, as well as extrinsic sources of nonlinearity, is an urgent requirement. A localized and strong rf magnetic field, created by a magnetic write head, is integrated into our nonlinear-Meissner-effect scanning microwave microscope [Tamin Tai, X. X. Xi, C. G. Zhuang, D. I. Mircea, and S. M. Anlage, IEEE Trans. Appl. Supercond. 21, 2615 (2011)]. MgB2 films with thickness 50 nm, fabricated by a hybrid physical-chemical vapor deposition technique on dielectric substrates, are measured at a fixed location and show a strongly temperature-dependent third harmonic response. We propose that several possible mechanisms are responsible for this nonlinear response.",1309.1706v1 2013-12-26,A Novel High-Pressure Monoclinic Metallic Phase of V2O3,"Vanadium sesquioxide, V2O3, is a prototypical metal-to-insulator system where, in temperature-dependent studies, the transition always coincides with a corundum-to-monoclinic structural transition. As a function of pressure, V2O3 follows the expected behavior of increased metallicity due to a larger bandwidth for pressures up to 12.5 GPa. Surprisingly, for higher pressures when the structure becomes unstable, the resistance starts to increase. Around 32.5 GPa at 300 K, we observe a novel pressure-induced corundum-to-monoclinic transition between two metallic phases, showing that the structural phase transition can be decoupled from the metal-insulator transition. Using X-ray Raman scattering, we find that screening effects, which are strong in the corundum phase, become weakened at high pressures. Theoretical calculations indicate that this can be related to a decrease in coherent quasiparticle strength, suggesting that the high-pressure phase is likely a critical correlated metal, on the verge of Mott-insulating behavior.",1312.7063v1 2014-06-19,Synthesis of SnTe Nanoplates with {100} and {111} Surfaces,"SnTe is a topological crystalline insulator that possesses spin-polarized, Dirac-dispersive surface states protected by crystal symmetry. Multiple surface states exist on the {100}, {110}, and {111} surfaces of SnTe, with the band structure of surface states depending on the mirror symmetry of a particular surface. Thus, to access surface states selectively, it is critical to control the morphology of SnTe such that only desired crystallographic surfaces are present. Here, we grow SnTe nanostructures using vapor-liquid-solid and vapor-solid growth mechanisms. Previously, SnTe nanowires and nanocrystals have been grown.1-4 In this report, we demonstrate synthesis of SnTe nanoplates with lateral dimensions spanning tens of microns and thicknesses of a hundred nanometers. The top and bottom surfaces are either (100) or (111), maximizing topological surface states on these surfaces. Magnetotransport on these SnTe nanoplates shows high bulk carrier density, consistent with bulk SnTe crystals arising due to defects such as Sn vacancies. In addition, we observe a structural phase transition in these nanoplates from the high temperature rock salt to low temperature rhombohedral structure. For nanoplates with very high carrier density, we observe a slight upturn in resistance at low temperatures, indicating electron-electron interactions.",1406.5227v1 2017-12-13,High Field (up to 140kOe) Angle Dependent Magneto Transport of Bi2Te3 Single Crystals,"We report the angle dependent high field (up to 140kOe) magneto transport of Bi2Te3 single crystals, a well-known topological insulator. The crystals were grown from melt of constituent elements via solid state reaction route by self-flux method. Details of crystal growth along with their brief characterization up to 5 Tesla applied field was reported by some of us recently [J. Magn. Mag. Mater. 428, 213 (2017)]. The angle dependence of the magneto-resistance (MR) of Bi2Te3 follows the cos Theta function i.e., MR is responsive, when the applied field is perpendicular (tilt angle Theta = o and/or 180) to the transport current. The low field (10 kOe) MR showed the signatures of weak anti localization (WAL) character with typical cusp near origin at 5 K. Further, the MR is linear right up to highest applied field of 140 kOe. The large positive MR are observed up to high temperatures and are above 250 and 150 percent at 140 kOe in perpendicular fields at 50 K and 100 K respectively. Heat capacity CP(T) measurements revealed the value of Debye temperature to be 135 K. ARPES (angle resolved photoemission spectroscopy) data clearly showed that the bulk Bi2Te3 single crystal consists of a single Dirac cone.",1712.04632v1 2018-05-14,Structural Dependence of Chemical Durability in Modified Aluminoborate Glasses,"Alkali and alkaline earth aluminoborate glasses feature high resistance to cracking under sharp contact loading compared to other oxide glasses. However, due to the high content of hygroscopic B2O3, it is expected that applications of these glasses could be hindered by poor chemical durability in aqueous solutions. Indeed, the compositional and structural dependence of their dissolution kinetics remains unexplored. In this work, we correlate the dissolution rates of aluminoborate glasses in acidic, neutral, and basic solutions with the structural changes induced by varying the aluminum-to-boron ratio. In detail, we investigate a total of seventeen magnesium, lithium, and sodium aluminoborate glasses with fixed modifier content of 25 mol%. We show that the structural changes induced by alumina depend on the network modifier. We also demonstrate a correlation between the chemical durability at various pH values and the structural changes in Mg-, Li- and Na- aluminoborate glasses. The substitution of alumina by boron oxide leads to a general decrease of chemical corrosion in neutral and acidic solutions. The lowest dissolution rate value is observed in Mg-aluminoborate glasses, as a consequence of the intermediate character of magnesium which can increase the network cross-linking. For basic solutions, the chemical durability is almost constant for the different amount of alumina in the three series, likely because B2O3 is susceptible to nucleophilic attack, which is favored in high-OH- solutions.",1805.05191v1 2018-06-12,Characterization of a depleted monolithic pixel sensors in 150 nm CMOS technology for the ATLAS Inner Tracker upgrade,"This work presents a depleted monolithic active pixel sensor (DMAPS) prototype manufactured in the LFoundry 150\,nm CMOS process. DMAPS exploit high voltage and/or high resistivity inclusion of modern CMOS technologies to achieve substantial depletion in the sensing volume. The described device, named LF-Monopix, was designed as a proof of concept of a fully monolithic sensor capable of operating in the environment of outer layers of the ATLAS Inner Tracker upgrade in 2025 for the High Luminosity Large Hadron Collider (HL-LHC). This type of devices has a lower production cost and lower material budget compared to presently used hybrid designs. In this work, the chip architecture will be described followed by the characterization of the different pre-amplifier and discriminator flavors with an external injection signal and an iron source (5.9\,keV x-rays).",1806.04400v1 2018-06-14,Demonstration of nonpolar m-plane vertical GaN-on-GaN p-n power diodes grown on free-standing GaN substrates,"This work demonstrates the first nonpolar vertical GaN on GaN pn power diodes grown on m-plane free standing substrates by MOCVD. The SEM and HRXRD results showed the good crystal quality of the homoepitaxial nonpolar structure with low defect densities. The CL result confirmed the nonpolar p GaN was of high quality with considerably reduced deep level states. At forward bias, the device showed good rectifying behaviors with a turn-on voltage of 4.0 V, an on-resistance of 2.3 mohmcm2, and a high on off ratio of 1e10. At reverse bias, the current leakage and breakdown were described by the trap assisted space charge limited current conduction mechanism, where I was proportional to V power 4.5. The critical electrical field was calculated to be 2.0 MV per cm without field plates or edge termination, which is the highest value reported on nonpolar power devices. The high performance m-plane p-n diodes can serve as key building blocks to further develop nonpolar GaN power electronics and polarization-engineering-related advanced power device structures for power conversion applications.",1806.05308v1 2019-09-23,Superconductivity up to 243 K in yttrium hydrides under high pressure,"The discovery of high-temperature conventional superconductivity in H3S with a critical temperature of Tc=203 K was followed by the recent record of Tc ~250 K in the face-centered cubic (fcc) lanthanum hydride LaH10 compound. It was realized in a new class of hydrogen-dominated compounds having a clathrate-like crystal structure in which hydrogen atoms form a 3D framework and surround a host atom of rare earth elements. Yttrium hydrides are predicted to have even higher Tc exceeding room temperature. In this paper, we synthesized and refined the crystal structure of new hydrides: YH4, YH6, and YH9 at pressures up to 237 GPa finding that YH4 crystalizes in the I4/mmm lattice, YH6 in Im-3m lattice and YH9 in P63/mmc lattice in excellent agreement with the calculations. The observed very high-temperature superconductivity is comparable to that found in fcc-LaH10: the pressure dependence of Tc for YH9 also displays a ""dome like shape"" with the highest Tc of 243 K at 201 GPa. We also observed a Tc of 227 K at 237 GPa for the YH6 phase. However, the measured Tcs are notably lower by ~30 K than predicted. Evidence for superconductivity includes the observation of zero electrical resistance, a decrease of Tc under an external magnetic field and an isotope effect. The theoretically predicted fcc YH10 with the promising highest Tc>300 K was not stabilized in our experiments under pressures up to 237 GPa.",1909.10482v1 2019-02-26,Modelling a Transition-Edge Sensor X-ray Microcalorimeter Linear Array for Compton Profile Measurements and Energy Dispersive Diffraction,"Transition-edge sensors are a type of superconducting detector that offers high energy resolution based on their sharp resistance-temperature feature in the superconducting-to-normal transition. TES X-ray microcalorimeters have typically been designed and used for spectroscopic applications. In this work, we present a design optimization for a TES X-ray microcalorimeter array for high-energy scattering and diffraction measurements. In particular, Compton scattering provides information about the electron momentum distribution, while energy dispersive diffraction provides structural information about dense engineering materials. Compton scattering and energy dispersive diffraction experiments must be conducted in the very hard X-ray regime (~ 100 keV), demanding a high X-ray stopping power in the detector; therefore, an absorber with a large heat capacity is needed in conjunction with the TES. In addition, both applications would benefit from an array composed of parallel strips. We present a design for a TES X-ray microcalorimeter optimized for such applications. In particular, we model the longitudinal position dependence due to the finite thermal diffusion time in the absorber.",1902.10047v2 2019-07-14,Current-Induced magnetization switching by the high spin Hall conductivity $α$-W,"The spin Hall effect originating from 5d heavy transition metal thin films such as Pt, Ta, and W is able to generate efficient spin-orbit torques that can switch adjacent magnetic layers. This mechanism can serve as an alternative to conventional spin-transfer torque for controlling next-generation magnetic memories. Among all 5d transition metals, W in its resistive amorphous phase typically shows the largest spin-orbit torque efficiency ~ 0.20-0.50. In contrast, its conductive and crystalline $\alpha$ phase possesses a significantly smaller efficiency ~ 0.03 and no spin-orbit torque switching has yet been realized using $\alpha$-W thin films as the spin Hall source. In this work, through a comprehensive study of high quality W/CoFeB/MgO and the reversed MgO/CoFeB/W magnetic heterostructures, we show that although amorphous-W has a greater spin-orbit torque efficiency, the spin Hall conductivity of $\alpha$-W ($|\sigma_{\operatorname{SH}}^{\alpha\operatorname{-W}}|=3.71\times10^{5}\operatorname{\Omega}^{-1}\operatorname{m}^{-1}$) is ~3.5 times larger than that of amorphous-W ($|\sigma_{\operatorname{SH}}^{\operatorname{amorphous-W}}|=1.05\times10^{5}\operatorname{\Omega}^{-1}\operatorname{m}^{-1}$). Moreover, we demonstrate spin-orbit torque driven magnetization switching using a MgO/CoFeB/$\alpha$-W heterostructure. Our findings suggest that the conductive and high spin Hall conductivity $\alpha$-W can be a potential candidate for future low power consumption spin-orbit torque memory applications.",1907.06192v1 2020-02-22,Electron irradiation on multilayer PdSe$_2$ field effect transistors,"Palladium diselenide (PdSe2) is a recently isolated layered material that has attracted a lot of interest for the pentagonal structure, the air stability and the electrical properties largely tunable by the number of layers. In this work, PdSe2 is used in the form of multilayer as the channel of back-gate field-effect transistors, which are studied under repeated electron irradiations. Source-drain Pd leads enable contacts with resistance below 350 kOhm um. The transistors exhibit a prevailing n-type conduction in high vacuum, which reversibly turns into ambipolar electric transport at atmospheric pressure. Irradiation by 10 keV electrons suppresses the channel conductance and promptly transforms the device from n-type to p-type. An electron fluence as low as 160 e-/nm2 dramatically change the transistor behavior demonstrating a high sensitivity of PdSe2 to electron irradiation. The sensitivity is lost after few exposures, that is a saturation condition is reached for fluence higher than 4000 e-/nm2. The damage induced by high electron fluence is irreversible as the device persist in the radiation-modified state for several hours, if kept in vacuum and at room temperature. With the support of numerical simulation, we explain such a behavior by electron-induced Se atom vacancy formation and charge trapping in slow trap states at the Si/SiO_2 interface.",2002.09785v1 2020-04-27,Recent advancements of the NEWS-G experiment,"NEWS-G (New Experiments With Spheres-Gas) is an experiment aiming to shine a light on the dark matter conundrum with a novel gaseous detector, the spherical proportional counter. It uses light gases, such as hydrogen, helium, and neon, as targets to expand dark matter searches to the sub-GeV/c$^{2}$ mass region. NEWS-G produced its first results with a 60 cm in diameter detector installed at LSM (France), excluding at 90% C.L. cross-sections above $4.4\cdot{10}^{37}$ cm$^{2}$ for dark matter candidates of 0.5 GeV/c$^{2}$ mass. Currently, a 140 cm in diameter detector is being built at LSM and a commissioning run is underway, prior to its installation at SNOLAB (Canada) at the end of the year. Presented here are developments incorporated in this new detector: a) sensor technologies using resistive materials and multi-anode read-out that allow high gain and high pressure operation; b) gas purification techniques to remove contaminants (H$_{2}$O, O$_{2}$); c) reduction of ${}^{210}$Pb induced background through copper electroforming methods; d) utilisation of UV-lasers for detector calibration, detector response monitoring and estimation of gas related fundamental properties. This next phase of NEWS-G will allow searches for low mass dark matter with unprecedented sensitivity.",2004.12795v1 2016-03-02,Conformal Titanium Nitride in a Porous Silicon Matrix: a Nanomaterial for In-Chip Supercapacitors,"Today's supercapacitor energy storages are typically discrete devices aimed for printed boards and power applications. The development of autonomous sensor networks and wearable electronics and the miniaturisation of mobile devices would benefit substantially from solutions in which the energy storage is integrated with the active device. Nanostructures based on porous silicon (PS) provide a route towards integration due to the very high inherent surface area to volume ratio and compatibility with microelectronics fabrication processes. Unfortunately, pristine PS has limited wettability and poor chemical stability in electrolytes and the high resistance of the PS matrix severely limits the power efficiency. In this work, we demonstrate that excellent wettability and electro-chemical properties in aqueous and organic electrolytes can be obtained by coating the PS matrix with an ultra-thin layer of titanium nitride by atomic layer deposition. Our approach leads to very high specific capacitance (15 F/cm$^3$), energy density (1.3 mWh/cm$^3$), power density (up to 214 W/cm$^3$) and excellent stability (more than 13,000 cycles). Furthermore, we show that the PS-TiN nanomaterial can be integrated inside a silicon chip monolithically by combining MEMS and nanofabrication techniques. This leads to realisation of in-chip supercapacitor, i.e., it opens a new way to exploit the otherwise inactive volume of a silicon chip to store energy.",1603.00798v1 2019-02-28,Effect of atomic ordering on the magnetic anisotropy of single crystal Ni80Fe20,"We investigate the effect of atomic ordering on the magnetic anisotropy of Ni80Fe20 at.% (Py). To this end, Py films were grown epitaxially on MgO (001) using dc magnetron sputtering (dcMS) and high power impulse magnetron sputtering (HiPIMS). Aside from twin boundaries observed in the latter case, both methods present high quality single crystals with cube-on-cube epitaxial relationship as verified by the polar mapping of important crystal planes. However, X-ray diffraction results indicate higher order for the dcMS deposited film towards L12 Ni3Fe superlattice. This difference can be understood by the very high deposition rate of HiPIMS during each pulse which suppresses adatom mobility and ordering. We show that the dcMS deposited film presents biaxial anisotropy while HiPIMS deposition gives well defined uniaxial anisotropy. Thus, higher order achieved in the dcMS deposition behaves as predicted by magnetocrystalline anisotropy i.e. easy axis along the [111] direction that forced in the plane along the [110] direction due to shape anisotropy. The uniaxial behaviour in HiPIMS deposited film then can be explained by pair ordering or more recent localized composition non-uniformity theories. Further, we studied magnetoresistance of the films along the [100] directions using an extended van der Pauw method. We find that the electrical resistivities of the dcMS deposited film are lower than in their HiPIMS counterparts verifying the higher order in the dcMS case.",1903.00105v1 2019-03-29,Multi-contact Phase Change Toggle Logic Device Utilizing Thermal Crosstalk,"Phase change memory (PCM) is an emerging high speed, high density, high endurance, and scalable non-volatile memory technology which utilizes the large resistivity contrast between the amorphous and crystalline phases of chalcogenide materials such as Ge2Sb2Te5 (GST). In addition to being used as a standalone memory, there has been a growing interest in integration of PCM devices on top of the CMOS layer for computation in memory and neuromorphic computing. The large CMOS overhead for memory controllers is a limiting factor for this purpose. Transferring functionality like routing, multiplexing, and logic to the memory layer can substantially reduce the CMOS overhead, making it possible to integrate 100s of GB of PCM storage on top of a conventional CPU. In this work, we present computational analysis of a phase change device concept that can perform toggle operations. The toggle functionality is achieved using two physical mechanisms: (i) isolation of different read contacts due to amorphization between different write contact pairs, and (ii) thermal cross-talk between a molten region and a previously amorphized region. Phase-change devices with six contacts can be implemented as toggle flip-flops, multiplexer, or demultiplexer when interfaced with CMOS transistors. Here, we demonstrate the operation of the device as a toggle flip-flop with 5 transistors, requiring ~50% of the footprint compared to conventional CMOS alternatives, with the added advantage of non-volatility.",1904.00836v1 2021-01-05,High-Temperature Superconductivity in Cerium Superhydrides,"The discoveries of high-temperature superconductivity in H3S and LaH10 have excited the search for superconductivity in compressed hydrides. In contrast to rapidly expanding theoretical studies, high-pressure experiments on hydride superconductors are expensive and technically challenging. Here we experimentally discover superconductivity in two new phases,Fm-3m-CeH10 (SC-I phase) and P63/mmc-CeH9 (SC-II phase) at pressures that are much lower (<100 GPa) than those needed to stabilize other polyhydride superconductors. Superconductivity was evidenced by a sharp drop of the electrical resistance to zero, and by the decrease of the critical temperature in deuterated samples and in an external magnetic field. SC-I has Tc=115 K at 95 GPa, showing expected decrease on further compression due to decrease of the electron-phonon coupling (EPC) coefficient {\lambda} (from 2.0 at 100 GPa to 0.8 at 200 GPa). SC-II has Tc = 57 K at 88 GPa, rapidly increasing to a maximum Tc ~100 K at 130 GPa, and then decreasing on further compression. This maximum of Tc is due to a maximum of {\lambda} at the phase transition from P63/mmc-CeH9 into a symmetry-broken modification C2/c-CeH9. The pressure-temperature conditions of synthesis affect the actual hydrogen content, and the actual value of Tc. Anomalously low pressures of stability of cerium superhydrides make them appealing for studies of superhydrides and for designing new superhydrides with even lower pressures of stability.",2101.01315v2 2015-07-30,Likelihood-free inference in high-dimensional models,"Methods that bypass analytical evaluations of the likelihood function have become an indispensable tool for statistical inference in many fields of science. These so-called likelihood-free methods rely on accepting and rejecting simulations based on summary statistics, which limits them to low dimensional models for which the absolute likelihood is large enough to result in manageable acceptance rates. To get around these issues, we introduce a novel, likelihood-free Markov-Chain Monte Carlo (MCMC) method combining two key innovations: updating only one parameter per iteration and accepting or rejecting this update based on subsets of statistics sufficient for this parameter. This increases acceptance rates dramatically, rendering this approach suitable even for models of very high dimensionality. We further derive that for linear models, a one dimensional combination of statistics per parameter is sufficient and can be found empirically with simulations. Finally, we demonstrate that our method readily scales to models of very high dimensionality using both toy models as well as by jointly inferring the effective population size, the distribution of fitness effects of new mutations (DFE) and selection coefficients for each locus from data of a recent experiment on the evolution of drug-resistance in Influenza.",1507.08612v2 2019-06-19,"Scalable, green fabrication of single-crystal noble metal films and nanostructures for low-loss nanotechnology applications","High quality metal thin films and nanostructures are critical building blocks for next generation nanotechnologies. They comprise low-loss circuit elements in nanodevices, provide new catalytic pathways for water splitting and $CO_2$ reduction technologies, and enable the confinement of spatially extended electromagnetic waves to be harnessed for application in information processing, energy harvesting, engineered metamaterials, and new technologies that will operate in the quantum plasmonics limit. However, the controlled fabrication of high-definition single-crystal subwavelength metal nanostructures remains a significant hurdle, due to the tendency for polycrystalline metal growth using conventional physical vapor deposition methods, and the challenges associated with placing solution-grown nanocrystals in desired orientations and locations on a surface to fabricate functional devices. Here, we introduce a new scalable, green, wet chemical approach to monocrystalline noble metals that enables the fabrication of ultrasmooth, epitaxial, single-crystal films of controllable thickness. They are ideal for the subtractive manufacture of nanostructure through ion beam milling, and additive crystalline nanostructure via lithographic patterning to enable large area, single-crystal metamaterials and high aspect ratio nanowires. Our single-crystal nanostructures demonstrate improved feature quality and pattern transfer yield, reduced optical and resistive losses, tailored local fields, and greatly improved stability compared to polycrystalline structures, supporting greater local field enhancements and enabling new practical advances at the nanoscale.",1906.07879v1 2019-10-23,Implications for Dark Matter Direct Detection in the Presence of LIGO-Motivated Primordial Black Holes,"We discuss formation of dark matter (DM) mini-halos around primordial black holes (PBHs) and its implication on DM direct detection experiments, including axion searches. Motivated by LIGO observations, we consider $f_{\textrm{DM}} \simeq 0.01$ as the fraction of DM in PBHs with masses $10 M_{\odot} - 70 M_{\odot}$. In this case, we expect the presence of dressed PBHs after Milky Way halo formation with mini-halo masses peaked around $M_{\textrm{halo}} \sim (50-55) M_{\textrm{PBH}}$. We analyze the effect of tidal forces acting on dressed PBHs within the Milky Way galaxy. In the solar neighborhood, the mini-halos are resistant against tidal disruption from the mean-field potential of the galaxy and encounters with stars, but they undergo a small level of disruption caused by disk shocking. The presence of mini-halos around LIGO-motivated PBHs today could reduce by half the local dark matter background. High-resolution simulations are encouraged. If the proposed scenario is realized, chances of direct detection of DM would decrease.",1910.10575v3 2020-06-24,Predicting the propensity for thermally activated $β$ events in metallic glasses via interpretable machine learning,"The elementary excitations in metallic glasses (MGs), i.e., $\beta$ processes that involve hopping between nearby sub-basins, underlie many unusual properties of the amorphous alloys. A high-efficacy prediction of the propensity for those activated processes from solely the atomic positions, however, has remained a daunting challenge. Recently, employing well-designed site environment descriptors and machine learning (ML), notable progress has been made in predicting the propensity for stress-activated $\beta$ processes (i.e., shear transformations) from the static structure. However, the complex tensorial stress field and direction-dependent activation would induce non-trivial noises in the data, limiting the accuracy of the structure-property mapping learned. Here, we focus on the thermally activated elementary excitations and generate high-quality data in several Cu-Zr MGs, allowing quantitative mapping of the potential energy landscape. After fingerprinting the atomic environment with short- and medium-range interstice distribution, ML can identify the atoms with strong resistance or high compliance to thermal activation, at an unprecedented accuracy over ML models for stress-driven activation events. Interestingly, a quantitative ""between-task"" transferring test reveals that our learnt model can also generalize to predict the propensity of shear transformation. Our dataset is potentially useful for benchmarking future ML models on structure-property relationships in MGs.",2006.13552v1 2020-10-07,Physical properties and electronic structure of single-crystal KCo$_2$As$_2$,"We present a method for producing high quality KCo2As2 crystals, stable in air and suitable for a variety of measurements. X-ray diffraction, magnetic susceptibility, electrical transport and heat capacity measurements confirm the high quality and an absence of long range magnetic order down to at least 2 K. Residual resistivity values approaching 0.25 $\mu\Omega$~cm are representative of the high quality and low impurity content, and a Sommerfeld coefficient $\gamma$ = 7.3 mJ/mol K$^2$ signifies weaker correlations than the Fe-based counterparts. Together with Hall effect measurements, angle-resolved photoemission experiments reveal a Fermi surface consisting of electron pockets at the center and corner of the Brillouin zone, in line with theoretical predictions and in contrast to the mixed carrier types of other pnictides with the ThCr2Si2 structure. A large, linear magnetoresistance of 200\% at 14~T, together with an observed linear and hyperbolic, rather than parabolic, band dispersions are unusual characteristics of this metallic compound and may indicate more complex underlying behavior.",2010.03447v2 2020-10-16,Investigation of n-type dilute magnetic semiconductor property observed in amorphous AlNO alloy thin film incorporated with dilute nitrogen at 300K,"In the present work, a thin film was deposited on quartz substrate by reactive RF magnetron sputtering of high purity (99.999%) aluminium target using ultra-high pure (Ar + N2) gas mixture. The percentage ratio of Ar and N2 in the gas mixture was 95% and 5%, respectively. Chemical characterization using x-ray photoelectron spectroscopy (XPS) and energy-dispersive xray (EDX) spectroscopy reveals that in the presence of dilute nitrogen, Al prefers to react with residual oxygen to form Al2O3 while the nitrogen is incorporated in it. The stoichiometry of bulk film is Al2N0.38O3.1. Magnetic and electrical properties measurement shows that the film exhibits ntype dilute magnetic semiconductor (DMS) property at 300K. The film has low electrical resistivity of 6.3 {\Omega}-cm and high carrier mobility of 5.7*106 cm2V-1s-1 at 300K. A density functional theory (DFT) calculation was performed to investigate the origin of observed magnetism in the film. From first-principles calculation based on DFT, it is found that for thermodynamic stability dilute nitrogen incorporated in Al2O3 preferred to sit at the interstitial site, which is responsible for observed magnetic property. Present study reported here provides a new insight to prepare rarely observed n-type DMS at room temperature by incorporating nitrogen interstitials in Al2O3, which is desirable for potential application in the field of spintronics.",2010.08361v1 2020-11-03,In situ mechanical testing of an Al matrix composite to investigate compressive plasticity and failure on multiple length scales,"SiC particle-reinforced Al matrix composites exhibit high strength, high wear resistance, and excellent high-temperature performance, but can also have low plasticity and fracture toughness, which limits their use in structural applications. This study investigates the plasticity and failure of such a composite on multiple length scales, from strain localization through a complex microstructure to the debonding of individual microparticles from the matrix. Three microscale pillars containing microstructures with different complexities and sizes/volume fraction of SiC particles were used to study the effect of these features on deformation. For the matrix, nanoscale intermetallic precipitates within the Al grains contribute most to the strengthening effect, and the Al grain boundaries are shown to be effective obstacles for preventing strain localization by dominant shear bands and, therefore, catastrophic failure. When shear localization occurs, SiC particles can then debond from the matrix if the shear band and interface are aligned. To investigate whether the interface is a weak point during catastrophic failure, a number of SiC particles were separated from the matrix with direct debonding tests, which yield an interface strength that is much higher than the critical resolved shear stress for a pillar exhibiting both shear localization and interface debonding. Therefore, the matrix-particle interface is ruled out as a possible weak point, and instead shear localization is identified as the mechanism that can drive subsequent interface debonding.",2011.01390v3 2020-12-04,"Revealing the Nanostructure of Mesoporous Fuel Cell Catalyst Supports for Durable, High-Power Performance","Achieving high power performance and durability with low Pt loadings are critical challenges for proton exchange membrane fuel cells. PtCo catalysts developed on new carbon black supports show promise by simultaneously providing good oxygen reduction kinetics and local oxygen transport. We investigate the role of nanoscale morphology in the performance of these catalysts supported on accessible (HSC-e and HSC-f) and conventional (Ketjen Black) porous carbons using 3D electron tomography, nitrogen sorption, and electrochemical performance measurements. We find that the accessible porous carbons have hollow interiors with mesopores that are larger and more numerous than conventional porous carbons. However, mesopore-sized openings (>2nm width) are too rare to account for significant oxygen transport. Instead we propose the primary oxygen transport pathway into the interior is through 1-2nm microporous channels permeating the carbon. The increased mesoporosity in the accessible porous carbons results in a shorter diffusion pathlength through constrictive, tortuous micropores in the support shell leading to lower local oxygen transport resistance. In durability testing, the accessible porous carbons show faster rates of electrochemical surface area loss, likely from fewer constrictive pores that would mitigate coarsening, but maintain superior high current density performance at end of life from the improved local oxygen transport.",2012.02879v1 2020-12-08,Complex impedance and Raman spectroscopy of Na$_{0.5}$(Bi$_{1-x}$Dy$_x$)$_{0.5}$TiO$_3$ ceramics,"In this work structural refinement, complex impedance spectroscopy, and Raman spectroscopy have been investigated on Na$_{0.5}$(Bi$_{1-x}$Dy$_x$)$_{0.5}$TiO$_3$ (xDyNBT) ceramic systems. The pure NBT, 2DyNBT and 5DyNBT compounds crystallize in a rhombohedral structure while the 15DyNBT composition crystallizes in an orthorhombic Pnma structure. We reported that dysprosium addition affects the phase transition temperatures as well as the dielectric losses. The electrical transport at high temperatures was investigated using the CIS over a wide frequency range. The studied samples showed a non-Debye type process, with a short-range relaxation for the pure NBT and a coexistence of both localized and long-range relaxations of charge carriers for the 2DyNBT and 5DyNBT compounds. For the high concentration, 15DyNBT, a short-range relaxation is observed. Moreover, using a brick-layer model we discuss the resistance and capacitance of the different contributors (grain and grain boundaries) in our samples. High temperature Raman spectroscopy investigation was performed in order to follow the temperature evolution of the structural transformations on ferroelectric compounds. Anomalies in the temperature evolution of the vibrational modes are seen to correlate well with the temperature transitions observed from dielectric measurements.",2012.04325v1 2021-02-18,Characterization of high aspect ratio TiAu TES X-ray microcalorimeters array using the X-IFU Frequency Domain Multiplexing readout,"We are developing X-ray microcalorimeters as a backup option for the baseline detectors in the X-IFU instrument on board the ATHENA space mission led by ESA and to be launched in the early 2030s.5$\times$5 mixed arrays with TiAu transition-edge sensor (TES), which have different high aspect ratios and thus high resistances, have been designed and fabricated to meet the energy resolution requirement of the X-IFU instrument. Such arrays can also be used to optimise the performance of the Frequency Domain Multiplexing (FDM) readout and lead to the final steps for the fabrication of a large detector array. In this work we present the experimental results from tens of the devices with an aspect ratio (length-to-width) ranging from 1-to-1 up to 6-to-1, measured in a single-pixel mode with a FDM readout system developed at SRON/VTT. We observed a nominal energy resolution of about 2.5 eV at 5.9 keV at bias frequencies ranging from 1 to 5 MHz. These detectors are proving to be the best TES microcalorimeters ever reported in Europe, being able to meet not only the requirements of the X-IFU instrument, but also those of other future challenging X-ray space missions, fundamental physics experiments, plasma characterization and material analysis.",2102.09378v1 2021-07-19,Miniaturization of Josephson junction for digital superconducting circuits,"In this work, we briefly overview various options for Josephson junctions which should be scalable down to nanometer range for utilization in nanoscale digital superconducting technology. Such junctions should possess high values of critical current, $I_c$, and normal state resistance, $R_n$. Another requirement is the high reproducibility of the junction parameters across a wafer in a fabrication process. We argue that Superconductor - Normal metal - Superconductor (SN-N-NS) Josephson junction of ""variable thickness bridge"" geometry is a promising choice to meet these requirements. Theoretical analysis of SN-N-NS junction is performed in the case where the distance between the S-electrodes is comparable to the coherence length of the N-material. The restriction on the junction geometrical parameters providing the existence of superconductivity in the S-electrodes is derived for the current flowing through the junction of an order of $I_c$. The junction heating, as well as available mechanisms for the heat removal, is analyzed. The obtained results show that an SN-N-NS junction with a high (sub-millivolt) value of $I_cR_n$ product can be fabricated from a broadly utilized combination of materials like Nb/Cu using well-established technological processes. The junction area can be scaled down to that of semiconductor transistors fabricated in the frame of a 40-nm process.",2107.08711v1 2021-11-18,Searching for Superconductivity in High Entropy Oxide Ruddlesden-Popper Cuprate Films,"In this work, the high entropy oxide A2CuO4 Ruddlesden-Popper (La0.2Pr0.2Nd0.2Sm0.2Eu0.2)2CuO4 is explored by charge doping with Ce+4 and Sr+2 at concentrations known to induce superconductivity in the simple parent compounds, Nd2CuO4 and La2CuO4. Electron doped (La0.185Pr0.185Nd0.185Sm0.185Eu0.185Ce0.075)2CuO4 and hole doped (La0.18Pr0.18Nd0.18Sm0.18Eu0.18Sr0.1)2CuO4 are synthesized and shown to be single crystal, epitaxially strained, and highly uniform. Transport measurements demonstrate that all as-grown films are insulating regardless of doping. Annealing studies show that resistivity can be tuned by modifying oxygen stoichiometry and inducing metallicity but without superconductivity. These results in turn are connected to extended x-ray absorption fine structure (EXAFS) results indicating that the lack of superconductivity in the high entropy cuprates likely originates from a large distortion within the Cu-O plane ({\sigma}2>0.015 {\AA}2) due to A-site cation size variance, which drives localization of charge carriers. These findings describe new opportunities for controlling charge- and orbital-mediated functional responses in Ruddlesden-Popper crystal structures, driven by balancing of cation size and charge variances that may be exploited for functionally important behaviors such as superconductivity, antiferromagnetism, and metal-insulator transitions, while opening less understood phase spaces hosting doped Mott insulators, strange metals, quantum criticality, pseudogaps, and ordered charge density waves.",2111.09767v1 2022-01-03,Phase Diagram of Infinite-layer Nickelate Compounds from First- and Second-principles Calculations,"The fundamental properties of infinite-layer rare-earth nickelates (RNiO2) are carefully revisited and compared with those of CaCuO2 and RNiO3 perovskites. Combining first-principles and finite-temperature second-principles calculations, we highlight that bulk NdNiO2 compound are far from equivalent to CaCuO2, together at the structural, electronic, and magnetic levels. Structurally, it is shown to be prone to spin-phonon coupling induced oxygen square rotation motion, which might be responsible for the intriguing upturn of the resistivity. At the electronic and magnetic levels, we point out orbital-selective Mott localization with strong out-of-plane band dispersion, which should result in the isotropic upper critical fields and weakly three-dimensional magnetic interactions with in-plane local moment and out-of-plane itinerant moment. We further demonstrate that as in RNiO3 perovskites, oxygen rotation motion and rare-earth ion controlled electronic and magnetic properties can give rise in RNiO2 compounds to a rich phase diagram and high tunability of various appealing properties. In line with that, we reveal that key ingredients of high-Tc superconductor such as orbital polarization, Fermi surface, and antiferromagnetic interactions can be deliberately controlled in NdNiO2 through epitaxial strain. Exploiting strain-orbital engineering, a crossover from three- to two-dimensional magnetic transition can be established, making then NdNiO2 thin film a true analog of high-Tc cuprates.",2201.00709v1 2022-03-20,Deposition temperature dependence of thermo-spin and magneto-thermoelectric conversion in Co$_2$MnGa films on Y$_3$Fe$_5$O$_{12}$ and Gd$_3$Ga$_5$O$_{12}$,"We have characterized Co$_2$MnGa (CMG) Heusler alloy films grown on Y$_3$Fe$_5$O$_{12}$ (YIG) and Gd$_3$Ga$_5$O$_{12}$ (GGG) substrates at different deposition temperatures and investigated thermo-spin and magneto-thermoelectric conversion properties by means of a lock-in thermography technique. X-ray diffraction, magnetization, and electrical transport measurements show that the deposition at high substrate temperatures induces the crystallized structures of CMG while the resistivity of the CMG films on YIG (GGG) prepared at and above 500 {\deg}C (550 {\deg}C) becomes too high to measure the thermo-spin and magneto-thermoelectric effects due to large roughness, highlighting the difficulty of fabricating highly ordered continuous CMG films on garnet structures. Our lock-in thermography measurements show that the deposition at high substrate temperatures results in an increase in the current-induced temperature change for CMG/GGG and a decrease in that for CMG/YIG. The former indicates the enhancement of the anomalous Ettingshausen effect in CMG through crystallization. The latter can be explained by the superposition of the anomalous Ettingshausen effect and the spin Peltier effect induced by the positive (negative) charge-to-spin conversion for the amorphous (crystallized) CMG films. These results provide a hint to construct spin-caloritronic devices based on Heusler alloys.",2203.10566v2 2022-04-10,Efficient route to achieve superconductivity improvement via substitutional La-Ce alloy superhydride at high pressure,"The discovery of clathrate superhydrides has approached the long-standing dream of room-temperature superconductivity and thus inspired their prosperous research under high pressure. However, how to experimentally optimize these compelling superhydrides is still a formidable challenge. Here, we find that half of the Ce atoms in the recently discovered hexagonal close packed (hcp) CeH9 structure can be randomly replaced by adjacent La, resulting in the formation of LaH9 unit that is impossible in a binary system. Our experiments show that hcp (La, Ce)H9 can be synthesized at ~110 GPa and possesses a maximum Tc of 178 K at higher pressure, which is evidenced by in-situ X-ray diffraction and electronic transport measurement where a sharp drop of resistivity to zero and a characteristic decrease of Tc under a magnetic field up to 9 T. More importantly, the Tc of (La, Ce)H9 is significantly increased by ~50-80 K compared to CeH9, showing the hitherto highest Tc at megabar pressure. Our experimental results not only verify the feasibility of improving the superconductivity of hydrides by introducing other suitable metals, but also provide important inspiration for finding high-Tc superconductors in various multinary superhydrides.",2204.04623v1 2022-06-16,A Lateral AlGaN/GaN Schottky Barrier Diode with 0.36 V Turn-on Voltage and 10 kV Breakdown Voltage by Using Double Barrier Anode Structure,"In this letter, we demonstrate a lateral AlGaN/GaN Schottky barrier diode (SBD) on sapphire substrate with low turn-on voltage (Von) and high breakdown voltage (VBK). By using a double barrier anode (DBA) structure formed by the mixture of Platinum (Pt) and Tantalum (Ta), the Von of the SBD can be as low as 0.36 V with a leakage current of 2.5E-6 A/mm. Supported by the high-quality carbon-doped GaN buffer on sapphire, the VBK can reach more than 10 kV with the anode-to-cathode spacing of 85 {\mu}m. Combining the VBK and the specific on-resistance (Ron,sp) of 25.1 m{\Omega}.cm^2, the power figure of merit of the SBD can reach 4.0 GW/cm^2, demonstrating a great potential for the application in ultra-high-voltage electronics.",2206.07881v1 2022-07-08,Synthesis and Superconductivity in yttrium superhydrides under high pressure,"The flourishing rare earth superhydrides are a class of recently discovered materials that possess near-room-temperature superconductivity at high pressures, opening a new era of superconductivity research at high pressures. Among these superhydrides, yttrium superhydrides attracted great interest owing to their abundance of stoichiometries and excellent superconductivities. Here, we carried out a comprehensive study of yttrium superhydrides in a wide pressure range of 145-300 GPa. We successfully synthesized a series of superhydrides with the compositions of YH4, YH6, YH7, and YH9, and reported their superconducting transition temperatures of 82 K at 167 GPa, 218 K at 165 GPa, 29 K at 162 GPa, and 230 K at 300 GPa, respectively, which were evidenced by a sharp drop of resistivity. The structure and superconductivity of YH4, which was taken as a representative example, were also examined by X-ray diffraction measurements and the suppression of the superconductivity under external magnetic fields, respectively. Clathrate YH10 as a candidate of room-temperature superconductor was not synthesized within the studied pressure and temperature ranges of up to 300 GPa and 2000 K, respectively. The current work created a detailed platform for further searching room-temperature superconductors in polynary yttrium-based superhydrides.",2207.03918v1 2022-08-31,Pouch cells with 15% silicon calendar-aged for 4 years,"Small amounts of high-capacity silicon-based materials are already used in the anode of commercial Li-ion batteries, helping increase their energy density. Despite their remarkable storage capability, silicon continuously reacts with the electrolyte, accelerating time-dependent cell performance fade. Nevertheless, very limited information is available on the specific consequences of this reactivity for the calendar aging of Li-ion cells. Here, we analyze aging effects on 450 mAh pouch cells containing 15 wt% of Si (and 73 wt% graphite) after storage at 21 oC for four years. We show that severe losses of Si capacity occurred due to particle isolation when cells were stored at high states of charge (SOC), but not when cells were fully discharged prior to storage. Impedance rise was also significantly higher when cells were kept at high SOCs and was mostly due to phenomena taking place at the cathode; the continuous electrolyte reduction at the anode did not lead to a major increase in bulk electrode resistance. A series of post-test characterization provided additional information on the effects of time and SOC on the calendar aging of Si-containing cells. Our study highlights the many challenges posed by Si during calendar aging and can inform future studies in the field.",2209.00138v1 2022-10-13,Diffusion mechanism and electrochemical investigation of 1T phase Al-MoS$_{2}$@rGO nano-composite as a high-performance anode for sodium-ion batteries,"We report the electrochemical investigation of 5% Al doped MoS$_2$@rGO composite as a high-performance anode for sodium (Na)-ion batteries. The x-ray diffraction (XRD), Raman spectroscopy and high-resolution transmission electron microscopy characterizations reveal that the Al doping increase the interlayer spacing of (002) plane of MoS$_2$ nanosheets and form a stable 1T phase. The galvanostatic charge-discharge measurements show the specific capacity stable around 450, 400, 350, 300 and 200 mAhg$^{-1}$ at current densities of 0.05, 0.1, 0.3, 0.5 and 1~Ag$^{-1}$, respectively. Also, we observe the capacity retentions of 86% and 66% at 0.1 and 0.3 Ag$^{-1}$, respectively, over 200 cycles with a consistent Coulombic efficiency of nearly 100%. The cyclic voltammetry, galvanostatic intermittent titration technique, and electrochemical impedance spectroscopy are used to find the kinetic behavior and the obtained value of diffusion coefficient falls in the range of 10$^{-10}$ to 10$^{-12}$ cm$^2$s$^{-1}$. Intriguingly, the in-situ EIS also explains the electrochemical kinetics of the electrode at different charge-discharge states with the variation of charge transfer resistance. Moreover, the post cycling investigation using ex-situ XRD and photoemission spectroscopy indicate the coexistence of 1T/2H phase and field-emission scanning electron microscopy confirm the stable morphology after 500 cycles. Also, the Na-ion transport properties are calculated for 1T Al--MoS$_2$@rGO interface and Al--MoS$_2$--MoS$_2$ interlayer host structure by theoretical calculations using density functional theory.",2210.06735v1 2022-11-02,Discovery of a high-temperature antiferromagnetic state and transport signatures of exchange interactions in a Bi2Se3/EuSe heterostructure,"Spatial confinement of electronic topological surface states (TSS) in topological insulators poses a formidable challenge because TSS are protected by time-reversal symmetry. In previous works formation of a gap in the electronic spectrum of TSS has been successfully demonstrated in topological insulator/magnetic material heterostructures, where ferromagnetic exchange interactions locally lifts the time-reversal symmetry. Here we report an experimental evidence of exchange interaction between a topological insulator Bi2Se3 and a magnetic insulator EuSe. Spin-polarized neutron reflectometry reveals a reduction of the in-plane magnetic susceptibility within a 2 nm interfacial layer of EuSe, and the combination of SQUID magnetometry and Hall measurements points to the formation of an antiferromagnetic layer with at least five-fold enhancement of N\'eel's temperature. Abrupt resistance changes in high magnetic fields indicate interfacial exchange coupling that affects transport in a TSS. High temperature local control of TSS with zero net magnetization unlocks new opportunities for the design of electronic, spintronic and quantum computation devices, ranging from quantization of Hall conductance in zero fields to spatial localization of non-Abelian excitations in superconducting topological qubits.",2211.01211v1 2022-11-09,Evolution of the strange-metal scattering in momentum space of electron-doped ${\rm La}_{2-x}{\rm Ce}_x{\rm CuO}_4$,"The linear-in-temperature resistivity is one of the important mysteries in the strange metal state of high-temperature cuprate superconductors. To uncover this anomalous property, the energy-momentum-dependent imaginary part of the self-energy Im ${\rm \Sigma}(k, \omega)$ holds the key information. Here we perform systematic doping, momentum, and temperature-dependent angle-resolved photoemission spectroscopy measurements of electron-doped cuprate ${\rm La}_{2-x}{\rm Ce}_x{\rm CuO}_4$ and extract the evolution of the strange metal scattering in momentum space. At low doping levels and low temperatures, Im ${\rm\Sigma} \propto \omega$ dependence dominates the whole momentum space. For high doping levels and high temperatures, Im ${\rm\Sigma} \propto \omega^2$ shows up, starting from the antinodal region. By comparing with the hole-doped cuprates ${\rm La}_{2-x}{\rm Sr}_x{\rm CuO}_4$ and ${\rm Bi}_2{\rm Sr}_2{\rm CaCu}_2{\rm O}_8$, we find a dichotomy of the scattering rate exists along the nodal and antinodal direction, which is ubiquitous in the cuprate family. Our work provides new insight into the strange metal state in cuprates.",2211.04833v1 2023-03-30,Physics-based bias-dependent compact modeling of 1/f noise in single- to few- layer 2D-FETs,"1/f noise is a critical figure of merit for the performance of transistors and circuits. For two-dimensional devices (2D-FETs), and especially for applications in the GHz range where short-channel FETs are required, velocity saturation (VS) effect can result in the reduction of 1/f noise at high longitudinal electric fields. A new physics-based compact model is for the first time introduced for single- to few- layer 2D-FETs in this study, precisely validating 1/f noise experiments for various types of devices. The proposed model mainly accounts for the measured 1/f noise bias dependence as the latter is defined by different physical mechanisms. Thus, analytical expressions are derived, valid in all regions of operation in contrast to conventional approaches available in literature so far, accounting for carrier number fluctuation (DN), mobility fluctuation (Dmu}) and contact resistance (DR) effects based on the underlying physics that rules these devices. DN mechanism due to trapping/detrapping together with an intense Coulomb scattering effect, dominates 1/f noise from medium to strong accumulation region while Dmu, is also demonstrated to modestly contribute in subthreshold region. DR can also be significant in very high carrier density. The VS induced reduction of 1/f noise measurements at high electric fields, is also remarkably captured by the model. The physical validity of the model can also assist in extracting credible conclusions when conducting comparisons between experimental data from devices with different materials or dielectrics.",2303.17162v1 2023-04-03,CVD Graphene Contacts for Lateral Heterostructure MoS${_2}$ Field Effect Transistors,"Intensive research is carried out on two-dimensional materials, in particular molybdenum disulfide, towards high-performance transistors for integrated circuits. Fabricating transistors with ohmic contacts is challenging due to the high Schottky barrier that severely limits the transistors' performance. Graphene-based heterostructures can be used in addition or as a substitute for unsuitable metals. We present lateral heterostructure transistors made of scalable chemical vapor-deposited molybdenum disulfide and chemical vapor-deposited graphene with low contact resistances of about 9 k${\Omega}$${\mu}$m and high on/off current ratios of 10${^8}$. We also present a theoretical model calibrated on our experiments showing further potential for scaling transistors and contact areas into the few nanometers range and the possibility of a strong performance enhancement by means of layer optimizations that would make transistors promising for use in future logic circuits.",2304.01177v2 2023-09-21,Superconductivity in Compositionally-Complex Cuprates with the YBa$_2$Cu$_3$O$_{7-x}$ Structure,"High-temperature superconductivity is reported in a series of compositionally-complex cuprates with varying degrees of size and spin disorder. Three compositions of Y-site alloyed YBa$_2$Cu$_3$O$_{7-x}$, i.e., (5Y)BCO, were prepared using solid-state methods with different sets of rare earth ions on the Y-site. Synchrotron X-ray diffraction and energy-dispersive X-ray spectroscopy confirm these samples have high phase-purity and homogeneous mixing of the Y-site elements. The superconducting phase transition was probed using electrical resistivity and AC magnetometry measurements, which reveal the transition temperature, T$_C$, is greater than 91 K for all series when near optimal oxygen doping. Importantly, these T$_C$ values are only $\approx$1$\%$ suppressed relative to pure YBCO (T$_C$ = 93 K). This result highlights the robustness of pairing in the YBCO structure to specific types of disorder. In addition, the chemical flexibility of compositionally-complex cuprates allows spin and lattice disorder to be decoupled to a degree not previously possible in high-temperature superconductors. This feature makes compositionally-complex cuprates a uniquely well-suited materials platform for studying proposed pairing interactions in cuprates.",2309.12535v1 2023-12-11,Local laser-induced solid-phase recrystallization of phosphorus-implanted Si/SiGe heterostructures for contacts below 4.2 K,"Si/SiGe heterostructures are of high interest for high mobility transistor and qubit applications, specifically for operations below 4.2 K. In order to optimize parameters such as charge mobility, built-in strain, electrostatic disorder, charge noise and valley splitting, these heterostructures require Ge concentration profiles close to mono-layer precision. Ohmic contacts to undoped heterostructures are usually facilitated by a global annealing step activating implanted dopants, but compromising the carefully engineered layer stack due to atom diffusion and strain relaxation in the active device region. We demonstrate a local laser-based annealing process for recrystallization of ion-implanted contacts in SiGe, greatly reducing the thermal load on the active device area. To quickly adapt this process to the constantly evolving heterostructures, we deploy a calibration procedure based exclusively on optical inspection at room-temperature. We measure the electron mobility and contact resistance of laser annealed Hall bars at temperatures below 4.2 K and obtain values similar or superior than that of a globally annealed reference samples. This highlights the usefulness of laser-based annealing to take full advantage of high-performance Si/SiGe heterostructures.",2312.06267v1 2023-03-13,Unusual magnetotransport and anomalous Hall effect in quasi-two-dimensional van der Waals ferromagnet Fe$_4$GeTe$_2$,"Fe$_4$GeTe$_2$, an itinerant vdW ferromagnet (FM) having Curie temperature (T$_C$) close to room temperature ($\sim 270$ K), exhibits another transition (T$_{SR}$ $\sim$ 120 K) where the easy axis of magnetization changes from in-plane to the out-of-plane direction in addition to T$_C$. Here, we have studied the magnetotransport in a multilayer Hall bar device fabricated on 300 nm Si/SiO$_2$ substrate. Interestingly, the zero field resistivity shows a negligible change in resistivity near T$_C$ unlike the typical metallic FM, whereas, it exhibits a dramatic fall below T$_{SR}$. Also, the resistivity shows a weak anomaly at T $ \sim $ 38 K (T$_Q$), below which the resistivity shows a quadratic temperature dependence according to the Fermi liquid behavior. Temperature-dependent Hall data exhibits important consequences. The ordinary Hall coefficient changes sign near T$_{SR}$ indicating the change in majority carriers. In a similar manner, the magnetoresistance (MR) data shows significantly large negative MR near T$_{SR}$ and becomes positive below T$_Q$. The observations of anomaly in the resistivity, sign-change of the ordinary Hall coefficient and maximum negative MR near T$_{SR}$, together suggest a possible Fermi surface reconstruction associated with the spin reorientation transition. Furthermore, analysis of the Hall data reveals a significant anomalous Hall conductivity (AHC) from $\sim 123 \Omega^{-1}$ cm$^{-1}$ (at T $\approx$ 5 K) to the maximum value of $\sim 366 \Omega^{-1}$ cm$^{-1}$ near T$_{SR}$. While the low-temperature part may originate due to the intrinsic KL mechanism, our analysis indicates that the temperature-dependent AHC is primarily appearing due to the side-jump mechanism as a result of the spin-flip electron-magnon scattering. Our study demonstrates an interplay between magnetism and band topology and its consequence on electron transport in Fe$_4$GeTe$_2$.",2303.07440v1 2020-03-04,Adaptive phase field modelling of crack propagation in orthotropic functionally graded materials,"In this work, we extend the recently proposed adaptive phase field method to model fracture in orthotropic functionally graded materials (FGMs). A recovery type error indicator combined with quadtree decomposition is employed for adaptive mesh refinement. The proposed approach is capable of capturing the fracture process with a localized mesh refinement that provides notable gains in computational efficiency. The implementation is validated against experimental data and other numerical experiments on orthotropic materials with different material orientations. The results reveal an increase in the stiffness and the maximum force with increasing material orientation angle. The study is then extended to the analysis of orthotropic FGMs. It is observed that, if the gradation in fracture properties is neglected, the material gradient plays a secondary role, with the fracture behaviour being dominated by the orthotropy of the material. However, when the toughness increases along the crack propagation path, a substantial gain in fracture resistance is observed.",2003.04689v1 2020-09-04,Impact of interfaces on the radiation response and underlying defect recovery mechanisms in nanostructured Cu-Fe-Ag,"Newest developments in nuclear fission and fusion technology as well as planned long-distance space missions demand novel materials to withstand harsh, irradiative environments. Radiation-induced hardening and embrittlement are a concern that can lead to failure of materials deployed in these applications. Here the underlying mechanisms are accommodation and clustering of lattice defects created by the incident radiation particles. Interfaces, such as free surfaces, phase and grain boundaries, are known for trapping and annihilating defects and therefore preventing these radiation-induced defects from forming clusters. In this work, differently structured nanocomposite materials based on Cu-Fe-Ag were fabricated using a novel solid-state route, combining severe plastic deformation with thermal and electrochemical treatments. The influence of different interface types and spacings on radiation effects in these materials was investigated using nanoindentation. Interface-rich bulk nanocomposites showed a slight decrease in hardness after irradiation, whereas the properties of a nanoporous material remain mostly unchanged. An explanation for this different material behavior and its link to recovery mechanisms at interfaces is attempted in this work, paving a concept towards radiation resistant materials.",2009.02039v1 2021-03-05,Effect of spoke design and material nonlinearity on non-pneumatic tire stiffness and durability performance,"Non-pneumatic tire has been widely used due to their advantages of no run-flat, no need of air maintenance, low rolling resistance, and improvement of passengers comfort due to its better shock absorption. It has variety of application in the military vehicle, earthmovers, lunar rover, stair climbing vehicles etc. Recently UPTIS (Unique Puncture-Proof Tire System) non pneumatic tire has been introduced for passenger vehicles. In this study three different design configuration Tweel, Honeycomb and newly developed UPTIS have been compared. Effect of Polyurethane (PU) material nonlinearity have also been introduced by applying 5 different nonlinear PU material property in the spokes. The combined analysis of the PU material nonlinearity and spoke design configuration on the overall tire stiffness and spoke damage prediction is analysed using 3-Dimensional FEM simulations performed in ANSYS 16.0. It has been observed that Mooney Rivlin 5-parameter model is best to capture all 5 studied PU materials the nonlinearity. Effect of material nonlinearity on various spoke designs have been studied. The best combination of spoke design and the use of nonlinear material have been suggested in terms of riding comfort, tire stiffness and durability performance.",2103.03637v1 2023-01-24,Seebeck-driven transverse thermoelectric generation in magnetic hybrid bulk materials,"The Seebeck-driven transverse thermoelectric generation in magnetic/thermoelectric hybrid materials (STTG) has been investigated in all-bulk hybrid materials. The transverse thermopower in a ferromagnetic Co$_2$MnGa/thermoelectric $n$-type Si hybrid bulk material with the adjusted dimensions reaches 16.0 $\mu$V/K at room temperature with the aid of the STTG contribution, which is much larger than the anomalous Nernst coefficient of the Co$_2$MnGa slab (6.8 $\mu$V/K). Although this transverse thermopower is smaller than the value for previously reported thin-film-based hybrid materials, the hybrid bulk materials exhibit much larger electrical power owing to their small internal resistance. This demonstration confirms the validity of STTG in bulk materials and clarifies its potential as a thermal energy harvester.",2301.09903v1 2023-01-24,Accelerate & Actualize: Can 2D Materials Bridge the Gap Between Neuromorphic Hardware and the Human Brain?,"Two-dimensional (2D) materials present an exciting opportunity for devices and systems beyond the von Neumann computing architecture paradigm due to their diversity of electronic structure, physical properties, and atomically-thin, van der Waals structures that enable ease of integration with conventional electronic materials and silicon-based hardware. All major classes of non-volatile memory (NVM) devices have been demonstrated using 2D materials, including their operation as synaptic devices for applications in neuromorphic computing hardware. Their atomically-thin structure, superior physical properties, i.e., mechanical strength, electrical and thermal conductivity, as well as gate-tunable electronic properties provide performance advantages and novel functionality in NVM devices and systems. However, device performance and variability as compared to incumbent materials and technology remain major concerns for real applications. Ultimately, the progress of 2D materials as a novel class of electronic materials and specifically their application in the area of neuromorphic electronics will depend on their scalable synthesis in thin-film form with desired crystal quality, defect density, and phase purity.",2301.10277v1 2023-07-19,Emergence of high-temperature superconducting phase in the pressurized La3Ni2O7 crystals,"The recent report of pressure-induced structure transition and signature of superconductivity with Tc = 80 K above 14 GPa in the La3Ni2O7 crystals has garnered considerable attention. To further elaborate this discovery, we carried out comprehensive resistance measurements on the La3Ni2O7 crystals grown with the optical-image floating zone furnace under oxygen pressure (15 bar) by using the diamond anvil cell (DAC) and cubic anvil cell (CAC), which employs the solid and liquid pressure transmitting medium, respectively. For the sample #1 measured in DAC, it exhibits a semiconducting-like behavior with large resistance at low pressures and becomes metallic gradually upon compression. At the pressures P >= 13.7 GPa, we observed the appearance of resistance drop as large as ~50% around 70 K, which evolves into a kink-like anomaly at pressures above 40 GPa and shifts to lower temperatures gradually with increasing magnetic field. These observations are consistent with the recent report mentioned above. On the other hand, the sample #2 measured in CAC retains the metallic behavior in the investigated pressure range up to 15 GPa. The hump-like anomaly in resistance around ~130 K at ambient pressure disappears at P >= 2 GPa. In the pressure range from 11 to 15 GPa, we observed the gradual development of a shoulder-like anomaly in resistance at low temperatures, which evolves into a pronounced drop of resistance by 98% below 62 K at 15 GPa, reaching a temperature-independent resistance of 20 uOhm below 20 K. Similarly, this resistance anomaly can be shifted to lower temperatures progressively by applying external magnetic fields, resembling a typical superconducting transition.",2307.09865v1 2023-07-27,High-temperature superconductivity with zero-resistance and strange metal behavior in La$_{3}$Ni$_{2}$O$_{7-δ}$,"Recently signatures of superconductivity were observed close to 80 K in \LN\ under pressure. This discovery positions \LN\ as the first bulk nickelate with high-temperature superconductivity, but the lack of zero resistance presents a significant drawback for validating the findings. Here we report pressure measurements up to over 30 GPa using a liquid pressure medium and show that single crystals of \LNO\ do exhibit zero resistance. We find that \LNO\ remains metallic under applied pressures, suggesting the absence of a metal-insulator transition proximate to the superconductivity. Analysis of the normal state $T$-linear resistance suggests an intricate link between this strange metal behaviour and superconductivity, whereby at high pressures both the linear resistance coefficient and superconducting transition are slowly suppressed by pressure, while at intermediate pressures both the superconductivity and strange metal behaviour appear disrupted, possibly due to a nearby structural instability. The association between strange metal behaviour and high-temperature superconductivity is very much in line with diverse classes of unconventional superconductors, including the cuprates and Fe-based superconductors. Understanding the superconductivity of \LNO\ evidently requires further revealing the interplay of strange metal behaviour, superconductivity, as well as possible competing electronic or structural phases.",2307.14819v2 2023-08-04,Stopping microfluidic flow,"We present a cross-comparison of three stop-flow configurations--such as low-pressure (LSF), high-pressure open-circuit (OC-HSF), and high-pressure short-circuit (SC-HSF) stop-flow--to rapidly bring a high flow velocity within a microchannel to a standstill. The average velocities inside the microchannels were reduced from > 1 m/s to < 10 um/s within 2s of initiating the stop-flow. The performance of the three stop-flow configurations was assessed by measuring the residual flow velocities within microchannels having three orders-of-magnitude different flow resistances. The LSF configuration outperformed the OC-HSF and SC-HSF configurations within the high flow resistance microchannel, and resulted in a residual velocity of < 10 um/s. The OC-HSF configuration resulted in a residual velocity of < 150 um/s within a low flow resistance microchannel. The SC-HSF configuration resulted in a residual velocity of < 200 um/s across the three orders-of-magnitude different flow resistance microchannels, and < 100 um/s for the low flow resistance channel. We hypothesized that the residual velocity resulted from the compliance in the fluidic circuit, which was further investigated by varying the elasticity of the microchannel walls and the connecting tubing. A numerical model was developed to estimate the expanded volumes of the compliant microchannel and connecting tubings under a pressure gradient and to calculate the distance traveled by the sample fluid. A comparison of the numerically and experimentally obtained traveling distances confirmed our hypothesis that the residual velocities were an outcome of the compliance in the fluidic circuit. Therefore, a configuration with minimal fluidic circuit compliance resulted in the least residual velocity.",2308.02386v2 2009-06-02,The Evolution of Gas Clouds Falling in the Magnetized Galactic Halo: High Velocity Clouds (HVCs) Originated in the Galactic Fountain,"In the Galactic fountain scenario, supernovae and/or stellar winds propel material into the Galactic halo. As the material cools, it condenses into clouds. By using FLASH three-dimensional magnetohydrodynamic simulations, we model and study the dynamical evolution of these gas clouds after they form and begin to fall toward the Galactic plane. In our simulations, we assume that the gas clouds form at a height of z=5 kpc above the Galactic midplane, then begin to fall from rest. We investigate how the cloud's evolution, dynamics, and interaction with the interstellar medium (ISM) are affected by the initial mass of the cloud. We find that clouds with sufficiently large initial densities (> 0.1 hydrogen atoms per cc) accelerate sufficiently and maintain sufficiently large column densities as to be observed and identified as high-velocity clouds (HVCs) even if the ISM is weakly magnetized (1.3 micro Gauss). We also investigate the effects of various possible magnetic field configurations. As expected, the ISM's resistance is greatest when the magnetic field is strong and perpendicular to the motion of the cloud. The trajectory of the cloud is guided by the magnetic field lines in cases where the magnetic field is oriented diagonal to the Galactic plane. The model cloud simulations show that the interactions between the cloud and the ISM can be understood via analogy to the shock tube problem which involves shock and rarefaction waves. We also discuss accelerated ambient gas, streamers of material ablated from the clouds, and the cloud's evolution from a sphere-shaped to a disk- or cigar-shaped object.",0906.0613v1 2018-10-30,THz-TDS time-trace analysis for the extraction of material and metamaterial parameters,"We report on a method and an associated open source software, Fit@TDS, working on an average personal computer. The method is based on the fitting of a time-trace data of a terahertz time-domain-spectroscopy system enabling the retrieval of the refractive index of a dielectric sample and the resonance parameters of a metasurface (quality factor, absorption losses, etc.). The software includes commonly used methods where the refractive index is extracted from frequency domain data. However, these methods are limited, for instance in case of a high noise level or when an absorption peak saturates the absorption spectrum bringing the signal to the noise level. Our software allows to use a new method where the refractive indices are directly fitted from the time-trace. The idea is to model a material or a metamaterial through parametric physical models (Drude-Lorentz model and time-domain coupled mode theory) and to implement the subsequent refractive index in the propagation model to simulate the time-trace. Then, an optimization algorithm is used to retrieve the parameters of the model corresponding to the studied material/metamaterial. In this paper, we explain the method and test it on fictitious samples to probe the feasibility and reliability of the proposed model. Finally, we used Fit@TDS on real samples of high resistivity silicon, lactose and gold metasurface on quartz to show the capacity of our method",1810.12567v4 2020-05-28,Graphene-TiS$_3$ heterojunction for selective polar vapor sensing at room temperature,"In this work, the room temperature polar vapor sensing behavior of two dimentional (2D) heterojunction Graphene-TiS3 materials and TiS3 nanoribbons is investigated. TiS3 nanoribbons were synthesized via chemical vapor transport (CVT) and their structure was investigated by scanning electron microscopy (SEM), high resolution transmission electron microscopy (HRTEM), energy dispersive X- ray spectroscopy (EDS), X-ray diffraction (XRD), Raman spectroscopy and Fourier transform infrared spectroscopy (FT-IR) analysis. The gas sensing performance of the TiS3 nanoribbons was assessed through the observed changes in their electronic behavior. Sensing devices were fabricated with gold contacts and with lithographically patterned graphene (Gr) electrodes in a 2D heterojunction Gr-TiS3-Gr architecture.. It is observed that the gold contacted TiS3 device has a rather linear I-V behavior while the Gr-TiS3-Gr heterojunction forms a contact with a higher Schottky barrier (250 meV). I-V responses of the sensors were recorded at room temperature with a relative humidity of 55% and for different ethanol vapor concentrations (varying from 2 to 20 ppm). I-V plots indicated an increase in the resistance of Gr-TiS3-Gr by the adsorption of water and ethanol molecules with relatively high sensing response (~3353% at 2 ppm). Our results reveal that selective and stable responses to a low concentration of ethanol vapor (2 ppm) can be achieved at room temperature with transient response and recovery times of around 6 s and 40 s, respectively. Our proposed design demonstrate a new approach for selective molecular recognition using polar interactions between analyte vapors and heterojunctions of 2D-materials.",2005.14245v1 2022-01-06,A quantitative assessment of Imaging High-Z and Medium-Z materials using Muon Scattering Tomography,"Muon Scattering Tomography (MST) has been shown to be a powerful technique for the non-invasive imaging of high-shielded objects. We present here the application of the MST technique to investigate two types of nuclear waste packages, a small-steel drum and a large nuclear waste cask, namely, a CASTOR V/52. We have developed a quantitative method using the contrast-to-noise ratio (CNR) to evaluate the performance of an MST detector system in differentiating between high-, medium-, and low-Z materials inside nuclear waste packages with different shielding types. This study reveals that our MST detector system is able to differentiate between a (10 $\times$ 10 $\times$ 10 cm$^3$) uranium cube, embedded within a concrete matrix inside the small-steel drum, and regions of background signal in six hours of muon exposure time with a CNR value of 3.1$\pm$0.2. During our investigation of the highly-shielded cask, the reconstructed images of the cask contents indicated the ability of our system to detect irregular baskets, such as empty baskets, with a CNR value of 5.0$\pm$0.3 after 30 days of muon exposure. These studies were done using a Monte Carlo simulation tuned to the performance of resistive plate chambers (RPCs) based muon tomography system built by the University of Bristol, which had a reported position resolution of 350 micron. Here we also report the dependence of the performance on the position resolution. We argue that using a combination of RPC and drift chambers (DC) detectors with 700 micron and 4 mm position resolutions respectively is able to generate tomographic images of well-shielded materials in a few hours of muon exposure time. With these position resolutions, our system needs six hours of muon exposure time to produce a good quality image of a cube of uranium with side-length of 10 cm shielded by a concrete matrix with CNR value of 2.4$\pm$0.25.",2201.01877v3 2023-03-07,Stacking disorder and thermal transport properties of $α$-RuCl$_3$,"$\alpha$-RuCl$_3$, a well-known candidate material for Kitaev quantum spin liquid, is prone to stacking disorder due to the weak van der Waals bonding between the honeycomb layers. After a decade of intensive experimental and theoretical studies, the detailed correlation between stacking degree of freedom, structure transition, magnetic and thermal transport properties remains unresolved. In this work, we reveal the effects of a small amount of stacking disorder inherent even in high quality $\alpha$-RuCl$_3$ crystals. This small amount of stacking disorder results in the variation of the magnetic ordering temperature, suppresses the structure transition and thermal conductivity. Crystals with minimal amount of stacking disorder have a T$_N>$7.4\,K and exhibit a well-defined structure transition around 140\,K upon cooling. For those with more stacking faults and a T$_N$ below 7\,K, the structure transition occurs well below 140\,K upon cooling and is incomplete, manifested by the diffuse streaks and the coexistence of both high temperature and low temperature phases down to the lowest measurement temperature. Both types of crystals exhibit oscillatory field dependent thermal conductivity and a plateau-like feature in thermal Hall resistivity in the field-induced quantum spin liquid state. However, $\alpha$-RuCl$_3$ crystals with minimal amount of stacking disorder have a higher thermal conductivity that pushes the thermal Hall conductivity to be closer to the half-integer quantized value. These findings demonstrate a strong correlation between layer stacking, structure transition, magnetic and thermal transport properties, underscoring the importance of interlayer coupling in $\alpha$-RuCl$_3$ despite the weak van der Waals bonding.",2303.03682v2 2023-12-27,"Combined effect of SiC and carbon on sintering kinetics, microstructure and mechanical properties of fine-grained binderless tungsten carbide","The study investigates the density, phase composition, microstructure and mechanical properties (microhardness, fracture toughness) of binderless WC + SiC and WC + SiC + C ceramics obtained by Spark Plasma Sintering (SPS). Nanopowders of a-WC produced by DC arc plasma chemical synthesis were used as raw materials. Powder compositions for sintering contained graphite (0.3, 0.5% wt.) or b-SiC (1, 3, 5% wt.) with 0.3% wt. graphite. It was shown that WC + 1% wt. SiC + 0.3% wt.C ceramics have a homogeneous fine-grained microstructure, high relative density, increased microhardness and Palmquist fracture toughness (Indentation Fracture Resistance). The kinetics of the initial sintering stage of WC + C and WC + C + SiC powder compositions was also analyzed using high-temperature dilatometry at the conventional pressureless sintering (CPS) conditions. The CPS and SPS activation energies of WC + SiC powder at the intensive shrinkage stage were determined using the Young-Cutler model. The CPS activation energies of WC, WC + C and WC + C + SiC powder compositions are close to the activation energy of diffusion of the carbon C along the a-WC grain boundaries. The SPS activation energies of WC + C and WC+ C + SiC powder compositions turn out to be lower than the activation energy of the C of a-WC grain boundary.",2312.16579v1 2022-07-26,Hysteresis-Free High Mobility Graphene Encapsulated in Tungsten Disulfide,"High mobility is a crucial requirement for a large variety of electronic device applications. The state-of-the-art for high quality graphene devices is based on heterostructures made with graphene encapsulated in $>80\,$nm-thick flakes of hexagonal boron nitride (hBN). Unfortunately, scaling up multilayer hBN while precisely controlling the number of layers remains an elusive challenge, resulting in a rough material unable to enhance the mobility of graphene. This leads to the pursuit of alternative, scalable materials, which can be simultaneously used as substrate and encapsulant for graphene. Tungsten disulfide (WS$_2$) is a transition metal dichalcogenide, which was successfully grown in large ($\sim$mm-size) multi-layers by chemical vapour deposition. However, the resistance \textit{vs} gate voltage characteristics when gating graphene through WS$_2$ exhibit largely hysteretic shifts of the charge neutrality point (CNP) in the order of $\Delta n\sim$2.6$\cdot$10$^{11}$ cm$^{-2}$, hindering the use of WS$_2$ as a reliable encapsulant. The hysteresis originates due to the charge traps from sulfur vacancies present in WS$_2$. In this work, we report for the first time the use of WS$_2$ as a substrate and the overcoming of hysteresis issues by chemically treating WS$_2$ with a super-acid, which passivates these vacancies and strips the surface from contaminants. The hysteresis is significantly reduced below the noise level by at least a factor five (to $\Delta n<$5$\cdot$10$^{10}$ cm$^{-2}$) and, simultaneously, the room-temperature mobility of WS$_2$-encapsulated graphene is as high as $\sim$6.2$\cdot$10$^{4}$ cm$^{-2}$V$^{-1}$s$^{-1}$ at a carrier density $n$ $\sim$1$\cdot$ 10$^{12}$ cm$^{-2}$. Our results promote WS$_2$ to a valid alternative to hBN as encapsulant for high-performance graphene devices.",2207.12836v1 2000-06-23,Temperature-Dependence of the Resistivity of a Dilute 2D Electron System in High Parallel Magnetic Field,"We report measurements of the resistance of silicon MOSFETs as a function of temperature in high parallel magnetic fields where the 2D system of electrons has been shown to be fully spin-polarized. A magnetic field suppresses the metallic behavior observed in the absence of a magnetic field. In a field of 10.8 T, insulating behavior is found for densities up to n_s approximately 1.35 x 10^{11} cm^{-2} or 1.5 n_c; above this density the resistance is a very weak function of temperature, varying less than 10% between 0.25 K and 1.90 K. At low densities the resistance goes to infinity more rapidly as the temperature is reduced than in zero field and the magnetoresistance diverges as T goes to 0.",0006379v4 2002-10-08,Resistivity of dilute 2D electrons in an undoped GaAs heterostructure,"We report resistivity measurements from 0.03 K to 10 K in a dilute high mobility 2D electron system. Using an undoped GaAs/AlGaAs heterojunction in a gated field-effect transistor geometry, a wide range of densities, $0.16 \times 10^{10} {cm}^{-2}$ to $7.5 \times 10^{10} {cm}^{-2}$, are explored. For high densities, the results are quantitatively shown to be due to scattering by acoustic phonons and impurities. In an intermediate range of densities, a peak in the resistivity is observed for temperatures below 1 K. This non-monotonic resistivity can be understood by considering the known scattering mechanisms of phonons, bulk and interface ionized impurities. Still lower densities appear insulating to the lowest temperature measured.",0210155v1 2003-09-11,Superconductivity on the localization threshold and magnetic-field-tuned superconductor-insulator transition in TiN films,"Temperature- and magnetic-field dependent measurements of the resistance of ultrathin superconducting TiN films are presented. The analysis of the temperature dependence of the zero field resistance indicates an underlying insulating behavior, when the contribution of Aslamasov-Larkin fluctuations is taken into account. This demonstrates the possibility of coexistence of the superconducting and insulating phases and of a direct transition from the one to the other. The scaling behavior of magnetic field data is in accordance with a superconductor-insulator transition (SIT) driven by quantum phase fluctuations in two-dimensional superconductor. The temperature dependence of the isomagnetic resistance data on the high-field side of the SIT has been analyzed and the presence of an insulating phase was confirmed. A transition from the insulating to a metallic phase is found at high magnetic fields, where the zero-temperature asymptotic value of the resistance being equal to h/e^2.",0309281v2 2003-10-02,Electrical resistivity of the Ti4O7 Magneli phase under high pressure,"We have measured resistivity as a function of temperature and pressure of Ti4O7 twinned crystals using different contact configurations. Pressures over 4kbar depress the localization of bipolarons and allow the study of the electrical conduction of the bipolaronic phase down to low temperatures. For pressures P > 40 kbar the bipolaron formation transition is suppressed and a nearly pressure independent behavior is obtained for the resistivity. We observed an anisotropic conduction. When current is injected parallel to the principal axis, a metallic conduction with interacting carrier effects is predominant. A superconducting state was not obtained down to 1.2 K, although evidences of the proximity of a quantum critical point were noticed. While when current is injected non-parallel to the crystal's principal axis, we obtained a logarithmic divergence of the resistivity at low temperatures. For this case, our results for the high pressure regime can be interpreted in the framework of interacting carriers (polarons or bipolarons) scattered by Two Level Systems.",0310048v1 2004-03-17,Interaction Correction to the Longitudinal Conductivity and Hall Resistivity in High Quality Two-Dimensional GaAs Electron and Hole Systems,"We present a systematic study of the corrections to both the longitudinal conductivity and Hall resistivity due to electron-electron interactions in high quality GaAs systems using the recent theory of Zala et al. [Phys. Rev. B 64, 214204 (2001)]. We demonstrate that the interaction corrections to the longitudinal conductivity and Hall resistivity predicted by the theory are consistent with each other. This suggests that the anomalous metallic drop in resistivity at B=0 is due to interaction effects and supports the theory of Zala et al.",0403411v1 2005-05-19,Universal scaling behavior of the c-axis resistivity of high-temperature superconductors,"We propose and show that the c-axis transport in high-temperature superconductors is controlled by the pseudogap energy and the c-axis resistivity satisfies a universal scaling law in the pseudogap phase. We derived approximately a scaling function for the c-axis resistivity and found that it fits well with the experimental data of Bi$_2$Sr$_2$CaCu$_2$O$_{8+\delta}$, Bi$_2$Sr$_2$Ca$_2$Cu$_3$O$_{10+\delta}$, and YBa$_2$Cu$_3$O$_{7-\delta}$. Our works reveals the physical origin of the semiconductor-like behavior of the c-axis resistivity and suggests that the c-axis hopping is predominantly coherent.",0505480v2 2006-07-27,Effect of DC electric field on longitudinal resistance of two dimensional electrons in a magnetic field,"The effect of a DC electric field on the longitudinal resistance of highly mobile two dimensional electrons in heavily doped GaAs quantum wells is studied at different magnetic fields and temperatures. Strong suppression of the resistance by the electric field is observed in magnetic fields at which the Landau quantization of electron motion occurs. The phenomenon survives at high temperature where Shubnikov de Haas oscillations are absent. The scale of the electric fields essential for the effect is found to be proportional to temperature in the low temperature limit. We suggest that the strong reduction of the longitudinal resistance is the result of a nontrivial change in the distribution function of 2D electrons induced by the DC electric field. Comparison of the data with recent theory yields the inelastic electron-electon scattering time $\tau_{in}$ and the quantum scattering time $\tau_q$ of 2D electrons at high temperatures, a regime where previous methods were not successful.",0607741v1 2009-05-07,Correlation between linear resistivity and Tc in organic and pnictide superconductors,"A linear temperature dependence of the electrical resistivity as T -> 0 is the hallmark of quantum criticality in heavy-fermion metals and the archetypal normal-state property of high-Tc superconductors, yet in both cases it remains unexplained. We report a linear resistivity on the border of spin-density-wave order in the organic superconductor (TMTSF)2X (X = PF6, ClO4), whose strength scales with the superconducting temperature Tc. This scaling, also present in the pnictide superconductors, reveals an intimate connection between linear-T scattering and pairing, shown by renormalization group theory to arise from antiferromagnetic fluctuations, enhanced by the interference of superconducting correlations. Our results suggest that linear resistivity in general may be a consequence of such interference and pairing in overdoped high-Tc cuprates is driven by antiferromagnetic fluctuations, as in organic and pnictide superconductors.",0905.0964v1 2010-02-25,Signatures of pressure induced superconductivity in insulating Bi2212,"We have performed several high pressure electrical resistance experiments on Bi1.98Sr2.06Y0.68Cu2O8, an insulating parent compound of the high-Tc Bi2212 family of copper oxide superconductors. We find a resistive anomaly, a downturn at low temperature, that onsets with applied pressure in the 20-40 kbar range. Through both resistance and magnetoresistance measurements, we identify this anomaly as a signature of induced superconductivity. Resistance to higher pressures decreases Tc, giving a maximum of 10 K. The higher pressure measurements exhibit a strong sensitivity to the hydrostaticity of the pressure environment. We make comparisons to the pressure induced superconductivity now ubiquitous in the iron arsenides.",1002.4672v1 2010-05-10,Analysis and Design of Ultra Thin Electromagnetic Absorbers Comprising Resistively Loaded High Impedance Surfaces,"High-Impedance Surfaces (HIS) comprising lossy Frequency Selective Surfaces (FSS) are employed to design thin electromagnetic absorbers. The structure, despite its typical resonant behavior, is able to perform a very wideband absorption in a reduced thickness. Losses in the frequency selective surface are introduced by printing the periodic pattern through resistive inks and hence avoiding the typical soldering of a large number of lumped resistors. The effect of the surface resistance of the FSS and dielectric substrate characteristics on the input impedance of the absorber is discussed by means of a circuital model. It is shown that the optimum value of surface resistance is affected both by substrate parameters (thickness and permittivity) and by FSS element shape. The equivalent circuit model is then used to introduce the working principles of the narrowband and the wideband absorbing structure and to derive the best-suited element for wideband absorption. Finally, the experimental validation of the presented structures is presented.",1005.1553v1 2011-07-05,Resistive Solutions for Pulsar Magnetospheres,"The current state of the art in the modeling of pulsar magnetospheres invokes either the vacuum or force-free limits for the magnetospheric plasma. Neither of these limits can simultaneously account for both the plasma currents and the accelerating electric fields that are needed to explain the morphology and spectra of high-energy emission from pulsars. To better understand the structure of such magnetospheres, we combine accelerating fields and force-free solutions by considering models of magnetospheres filled with resistive plasma. We formulate Ohm's Law in the minimal velocity fluid frame and construct a family of resistive solutions that smoothly bridges the gap between the vacuum and the force-free magnetosphere solutions. The spin-down luminosity, open field line potential drop, and the fraction of open field lines all transition between the vacuum and force-free values as the plasma conductivity varies from zero to infinity. For fixed inclination angle, we find that the spin-down luminosity depends linearly on the open field line potential drop. We consider the implications of our resistive solutions for the spin down of intermittent pulsars and sub-pulse drift phenomena in radio pulsars.",1107.0979v2 2011-11-02,Development and Performance of spark-resistant Micromegas Detectors,"The Muon ATLAS MicroMegas Activity (MAMMA) focuses on the development and testing of large-area muon detectors based on the bulk-Micromegas technology. These detectors are candidates for the upgrade of the ATLAS Muon System in view of the luminosity upgrade of Large Hadron Collider at CERN (sLHC). They will combine trigger and precision measurement capability in a single device. A novel protection scheme using resistive strips above the readout electrode has been developed. The response and sparking properties of resistive Micromegas detectors were successfully tested in a mixed (neutron and gamma) high radiation field, in a X-ray test facility, in hadron beams, and in the ATLAS cavern. Finally, we introduced a 2-dimensional readout structure in the resistive Micromegas and studied the detector response with X-rays.",1111.0426v1 2011-11-09,Nonequilibrium phenomena in high Landau levels,"Developments in the physics of 2D electron systems during the last decade have revealed a new class of nonequilibrium phenomena in the presence of a moderately strong magnetic field. The hallmark of these phenomena is magnetoresistance oscillations generated by the external forces that drive the electron system out of equilibrium. The rich set of dramatic phenomena of this kind, discovered in high mobility semiconductor nanostructures, includes, in particular, microwave radiation-induced resistance oscillations and zero-resistance states, as well as Hall field-induced resistance oscillations and associated zero-differential resistance states. We review the experimental manifestations of these phenomena and the unified theoretical framework for describing them in terms of a quantum kinetic equation. The survey contains also a thorough discussion of the magnetotransport properties of 2D electrons in the linear response regime, as well as an outlook on future directions, including related nonequilibrium phenomena in other 2D electron systems.",1111.2176v3 2011-12-12,Resistivity Calculations for Cuprate Superconductor Systems using an Electronic Phase Separation,"The resistivity as function of temperature of high temperature superconductors is very unusual and despite its importance lacks an unified theoretical explanation. It is linear with the temperature for overdoped compounds but it falls more quickly as the doping level decreases, and for weakly doped samples it has a minimum, increases like an insulator before it drops to zero at low temperatures. We show that this overall behavior can be explained by calculations using an electronic phase segregation into two main component phases with low and high densities. The total resistivity is calculated by the various contributions through several random picking processes of the local resistivities and using the Random Resistor Network approach.",1112.2631v1 2017-11-19,Global current circuit structure in a resistive pulsar magnetosphere model,"Pulsar magnetospheres have strong magnetic fields and large amounts of plasma. The structures of these magnetospheres are studied using force-free electrodynamics. To understand pulsar magnetospheres, discussions must include their outer region. However, force-free electrodynamics is limited in it does not handle dissipation. Therefore, a resistive pulsar magnetic field model is needed. To break the ideal magnetohydrodynamic (MHD) condition $E \cdot B = 0$, Ohm's law is used. In this work, I introduce resistivity depending upon the distance from the star and obtain a self-consistent steady state by time integration. Poloidal current circuits form in the magnetosphere while the toroidal magnetic-field region expands beyond the light cylinder and the Poynting flux radiation appears. High electric resistivity causes a large space scale poloidal current circuit and the magnetosphere radiates a larger Poynting flux than the linear increase outside of the light cylinder radius. The formed poloidal current circuit has width, which grows with the electric conductivity. This result contributes to a more concrete dissipative pulsar magnetosphere model.",1711.07471v1 2018-10-10,Test particles in relativistic resistive magnetohydrodynamics,"The Black Hole Accretion Code (BHAC) has recently been extended with the ability to evolve charged test particles according to the Lorentz force within resistive relativistic magnetohydrodynamics simulations. We apply this method to evolve particles in a reconnecting current sheet that forms due to the coalescence of two magnetic flux tubes in 2D Minkowski spacetime. This is the first analysis of charged test particle evolution in resistive relativistic magnetohydrodynamics simulations. The energy distributions of an ensemble of 100.000 electrons are analyzed, as well as the acceleration of particles in the plasmoids that form in the reconnection layer. The effect of the Lundquist number, magnetization, and plasma-$\beta$ on the particle energy distribution is explored for a range of astrophysically relevant parameters. We find that electrons accelerate to non-thermal energies in the thin current sheets in all cases. We find two separate acceleration regimes: An exponential increase of the Lorentz factor during the island coalescence where the acceleration depends linearly on the resistivity and a nonlinear phase with high variability. These results are relevant for determining energy distributions and acceleration sites obtaining radiation maps in large-scale magnetohydrodynamics simulations of black hole accretion disks and jets.",1810.04323v2 2019-07-07,"First demonstration of 200, 100, and 50 um pitch Resistive AC-Coupled Silicon Detectors (RSD) with 100% fill-factor for 4D particle tracking","We designed, produced, and tested RSD (Resistive AC-Coupled Silicon Detectors) devices, an evolution of the standard LGAD (Low-Gain Avalanche Diode) technology where a resistive n-type implant and a coupling dielectric layer have been implemented. The first feature works as a resistive sheet, freezing the multiplied charges, while the second one acts as a capacitive coupling for readout pads. We succeeded in the challenging goal of obtaining very fine pitch (50, 100, and 200 um) while maintaining the signal waveforms suitable for high timing and 4D-tracking performances, as in the standard LGAD-based devices.",1907.03314v3 2020-09-01,On resistive spiking of fungi,"We study long-term electrical resistance dynamics in mycelium and fruit bodies of oyster fungi P. ostreatus. A nearly homogeneous sheet of mycelium on the surface of a growth substrate exhibits trains of resistance spikes. The average width of spikes is c.~23~min and the average amplitude is c.~1~kOhm. The distance between neighbouring spikes in a train of spikes is c.~30~min. Typically there are 4-6 spikes in a train of spikes. Two types of resistance spikes trains are found in fruit bodies: low frequency and high amplitude (28~min spike width, 1.6~kOhm amplitude, 57~min distance between spikes) and high frequency and low amplitude (10~min width, 0.6~kOhm amplitude, 44~min distance between spikes). The findings could be applied in monitoring of physiological states of fungi and future development of living electronic devices and sensors.",2009.00292v1 2020-09-21,Contact resistance assessment and high-frequency performance projection of black phosphorus field-effect transistor technologies,"In this work, an evaluation of the contact quality of black phosphorus (BP) field-effect transistors (FETs) from different technologies previously reported is performed by means of an efficient and reliable contact resistance extraction methodology based on individual device practical characteristics. A good agreement is achieved between the extracted values with the Y-function method used here and reference values obtained with other methods considering internal values as well as with more expensive methods involving fabricated test structures. The method enables a direct evaluation of different steps in the same technology and it embraces the temperature dependence of the contact characteristics. Channel phenomena have no impact on the extracted contact resistance values. High-frequency performance projections are obtained for fabricated devices based on the extracted contact resistance.",2009.09661v3 2012-06-25,Performances of silicone coated high resistive bakelite RPC,"Performances of several single gap (gas gap 2 mm) prototype Resistive Plate Chambers (RPC) made of high resistive ({\rho} \sim 1010 - 1012 {\Omega} cm) bakelite, commercially available in India have been studied in recent times. To make the inner electrode surfaces smooth, a thin coating of silicone has been applied. An efficiency > 90% and time resolution \sim 2 ns (FWHM) have been obtained for both the streamer and the avalanche mode. The induced charge distributions of those silicone coated RPC are studied and the results are presented. A numerical study on the effect of surface roughness of the resistive electrodes on the electric field of the device has been carried out using Garfield-neBEM code. A few results for a simplified model representing surface roughness, measured using a surface profilometer for the bakelite surfaces, have also been presented.",1206.5627v1 2022-08-18,Observation of Fermi liquid phase with broken symmetry in a single crystalline nanorod of Pr$_2$Ir$_2$O$_7$,"We report experimental evidence of emergent broken symmetry Fermi liquid state in an isolated single crystalline nanorod of $\rm Pr_2 Ir_2 O_7$. We find clear signature of the onset of the Fermi liquid behavior at low temperature marked by the sign inversion of magnetoresistance from negative at high temperature, characteristic of incoherent Kondo scattering, to positive as well as a $\rm T^2$ dependence of resistivity at low temperature. A resistive anomaly is observed, which is accompanied by thermal hysteresis in the presence of magnetic field, suggesting itinerant metamagnetism. The observed high field negative magnetoresistance with quadratic field dependence at low temperature, which is most likely due to suppression of itinerant spin fluctuation, and the irreversibility of the magneto-resistive properties in the Fermi liquid regime suggest existence of an unusual state with broken spin rotation and time reversal symmetry, hallmark of `hastatic' order. The major features of such temperature dependence of resistivity and magnetoresistance can be explained in a phenomenological model incorporating two distinct hybridization channels, which is physically consistent with the possibility of the formation of the `hastatic' Fermi liquid phase.",2208.08811v1 2022-09-16,Prediction of Cross-Fitness for Adaptive Evolution to Different Environmental Conditions: Consequence of Phenotypic Dimensional Reduction,"How adaptive evolution to one environmental stress improves or suppresses adaptation to another is an important problem in evolutionary biology. For instance, in microbiology, the evolution of bacteria to be resistant to different antibiotics is a critical issue that has been investigated as cross-resistance. In fact, recent experiments on bacteria have suggested that the cross-resistance of their evolution to various stressful environments can be predicted by the changes to their transcriptome upon application of stress. However, there are no studies so far that explain a possible theoretical relationship between cross-resistance and changes in the transcriptome, which causes high-dimensional changes to cell phenotype. Here, we show that a correlation exists between fitness change in stress tolerance evolution and response to the environment, using a cellular model with a high-dimensional phenotype and establishing the relationship theoretically. The present results allow for the prediction of evolution from transcriptome information in response to different stresses before evolution. The relevance of this to microbiological evolution experiments is discussed.",2209.07756v2 2023-09-29,Pressure-induced superconductivity in polycrystalline La3Ni2O7,"We synthesized polycrystalline La3Ni2O7 samples by using the sol-gel method without post-annealing under high oxygen pressure, and then measured temperature-dependent resistivity under various hydrostatic pressures up to 14.5 GPa in a cubic anvil cell apparatus. We find that the density-wave-like anomaly in resistivity is progressively suppressed with increasing pressure and the resistivity drop corresponding to the onset of superconductivity emerges at pressure as low as 7 GPa. Zero resistivity is achieved at 9 GPa below 6.6 K, which increases quickly with pressure to 35.6 K at 14.5 GPa. The observation of zero-resistance state in the polycrystalline La3Ni2O7 samples under high pressures not only corroborates the recent report of superconductivity in the pressurized La3Ni2O7 crystals but also facilitates further studies on this emerging family of nickelate high-Tc superconductors.",2309.17378v2 2005-10-12,Magnetodielectric effect without multiferroic coupling,"The existence of a magnetodielectric (magnetocapacitance) effect is often used as a test for multiferroic behavior in new material systems. However, strong magnetodielectric effects can also be achieved through a combination of magnetoresistance and the Maxwell-Wagner effect, unrelated to multiferroic coupling. The fact that this resistive magnetocapacitance does not require multiferroic materials may be advantageous for some practical applications. Conversely, it also implies that magnetocapacitance per se is not sufficient to establish multiferroic coupling.",0510313v1 2007-09-24,External Control of a Metal-Insulator Transition in GaMnAs Wires,"Quantum transport in disordered ferromagnetic (III,Mn)V semiconductors is studied theoretically. Mesoscopic wires exhibit an Anderson disorder-induced metal-insulator transition that can be controlled by a weak external magnetic field. This metal-insulator transition should also occur in other materials with large anisotropic magneto resistance effects. The transition can be useful for studies of zero-temperature quantum critical phase transitions and fundamental material properties.",0709.3847v2 2008-01-28,Evidence for hyperconductivity and thermal superconductivity,"Physical explanation of hyperconductivity and thermal superconductivity existence is done in given article on the basis of inherent atomic nuclei oscillations in atoms of materials which are connected with electrons and phonons and in accordance with the well known Bardeen-Cooper-Schrieffer superconductivity theory. It is shown that hyperconductivity is the self-supporting, independent physical phenomenon which is caused by oscillations of atomic nuclei in atoms of materials and the minimal temperature of its existence does not reach absolute zero temperature. Hyperconductivity represents the typical dynamic condition of a material with zero electrical and zero thermal resistances.",0801.4212v1 2009-11-24,The possible superconductivity at 109 K in YBaCuO materials,"The new YBaCuO superconductors are synthesized by using the standard solid state reaction method as Y5-6-11, Y7-9-16, Y5-8-13, Y7-11-18, Y156, Y3-8-11, and Y13-20-23. We find that all material obtained are shown the Meissner effect at 77 K. The resistivity measurements are used by the four-probe method .The Y 7-11-18 has the highest onset as 109 K . The XRD spectra are shown that they have the same crystal structure as Y123 with some impurities peaks .",0911.4524v1 2012-12-20,Thermoelectricity in ternary rare-earth systems,"Crystallographic data, Seebeck coefficient, electrical resistance and thermal conductivity are reported for a large number of rare-earth compounds, manifestations of the Kondo effect being discussed. In more detail, thermoelectric properties of Yb3Co4Ge13 and Yb3Co4Sn13 compounds and Yb2CeCo4Ge13 and Yb2.3La0.7Co4Ge13 solid solutions are presented.",1212.4995v1 2015-05-07,Computer modelling of hafnium doping in lithium niobate,"Lithium niobate, LiNbO3, is an important technological material with good electro-optic, acousto-optic, elasto-optic, piezoelectric and nonlinear properties. Doping LiNbO3 with hafnium, Hf has been shown to improve the resistance of the material to optical damage. Computer modelling provides a useful means of determining the properties of doped and undoped LiNbO3, including its defect chemistry, and the effect of doping on the structure. In this paper, Hf doped LiNbO3 has been modelled, and the final defect configurations are found to be consistent with experimental results.",1505.01661v2 2022-11-24,"Anisotropic magnetoresistance: materials, models and applications","Resistance of certain (conductive and otherwise isotropic) ferromagnets turns out to exhibit anisotropy with respect to the direction of magnetisation: R$_\parallel$ different from R$_\perp$ with reference to the electric current direction. This century-old phenomenon is reviewed both from the perspective of materials and physical mechanisms involved. More recently, this effect has also been extended to antiferromagnets. This opens the possibility for industrial applications reaching far beyond the current ones, e.g. hard drive read heads or position sensors.",2212.03700v2 2024-05-15,The Detection of Unconventional Quantum Oscillations in Insulating 2D Materials,"In strongly correlated quantum materials, electrons behave in ways that often extend beyond the confines of conventional Fermi-liquid theory. Interesting results include the observation of low-temperature metallic behavior in systems that are highly resistive. Here we provide an overview of experiments in which insulators exhibit characteristics of a metal such as the Shubnikov de Haas like quantum oscillations, focusing on recent findings in the correlated insulating states of two-dimensional WTe2. We discuss the status of current research, clarify the debates and challenges in interpreting the experiments, rule out extrinsic explanations and discuss promising future directions.",2405.09666v2 1998-06-30,"Transport, optical and electronic properties of the half metal CrO2","The electronic structure of CrO_2 is critically discussed in terms of the relation of existing experimental data and well converged LSDA and GGA calculations of the electronic structure and transport properties of this half metal magnet, with a particular emphasis on optical properties. We find only moderate manifestations of many body effects. Renormalization of the density of states is not large and is in the typical for transition metals range. We find substantial deviations from Drude behavior in the far-infrared optical conductivity. These appear because of the unusually low energy of interband optical transitions. The calculated mass renormalization is found to be rather sensitive to the exchange-correlation functional used and varies from 10% (LSDA) to 90% (GGA), using the latest specific heat data. We also find that dressing of the electrons by spin fluctuations, because of their high energy, renormalizes the interband optical transition at as high as 4 eV by about 20%. Although we find no clear indications of strong correlations of the Hubbard type, strong electron-magnon scattering related to the half metallic band structure is present and this leads to a nontrivial temperature dependence of the resistivity and some renormalization of the electron spectra.",9806378v1 2002-08-14,Nonlinear microwave response of epitaxial YBaCuO films of varying oxygen content on MgO substrates,"We have investigated the nonlinear microwave properties of electron-beam coevaporated YBaCuO films on MgO, using stripline resonators at 2.3 GHz and temperatures 1.7-80 K. The oxygen content of the films ranged from strongly underdoped to overdoped. Above 20 K, the nonlinear response of the resonators was dominated by the superconductor. We could establish clear correlations between the nonlinear surface resistance, two-tone intermodulation (IMD), and oxygen content of the films, which indicate that the superconducting order parameter is important for the nonlinearities. An exponential rather than a power-law representation of the nonlinear current-voltage relation would be required to explain our results phenomenologically. Below 20 K, the dielectric loss tangent of MgO dominated the nonlinear response of the resonators. With increasing power, the dissipation losses decreased markedly, accompanied by enhanced IMD. The surface reactance passed through a shallow minimum at about 5 K, independent of power. We attribute these effects to resonant absorption by impurity states in MgO.",0208285v1 2004-04-13,"Quantum Transparency of Anderson Insulator Junctions: Statistics of Transmission Eigenvalues, Shot Noise, and Proximity Conductance","We investigate quantum transport through strongly disordered barriers, made of a material with exceptionally high resistivity that behaves as an Anderson insulator or a ``bad metal'' in the bulk, by analyzing the distribution of Landauer transmission eigenvalues for a junction where such barrier is attached to two clean metallic leads. We find that scaling of the transmission eigenvalue distribution with the junction thickness (starting from the single interface limit) always predicts a non-zero probability to find high transmission channels even in relatively thick barriers. Using this distribution, we compute the zero frequency shot noise power (as well as its sample-to-sample fluctuations) and demonstrate how it provides a single number characterization of non-trivial transmission properties of different types of disordered barriers. The appearance of open conducting channels, whose transmission eigenvalue is close to one, and corresponding violent mesoscopic fluctuations of transport quantities explain at least some of the peculiar zero-bias anomalies in the Anderson-insulator/superconductor junctions observed in recent experiments [Phys. Rev. B {\bf 61}, 13037 (2000)]. Our findings are also relevant for the understanding of the role of defects that can undermine quality of thin tunnel barriers made of conventional band-insulators.",0404271v2 2004-06-17,Phase formation of polycrystalline MgB2 at low temperature using nanometer Mg powder,"The MgB2 superconductor synthesized in a flowing argon atmosphere using nanometer magnesium powder as the raw materials, denoted as Nano-MgB2, has been studied by the technique of in-situ high temperature resistance measurement (HT-RT measurement). The MgB2 phase is identified to form within the temperature range of 430 to 490 C, which is much lower than that with the MgB2 sample fabricated in the same gas environment using the micron-sized magnesium powder, denoted as Micro-MgB2, reported previously. The sample density of the Nano-MgB2 reaches 1.7 g/cm3 with a crystal porosity structure less than a micrometer, as determined by the scanning electron microscope (SEM) images, while the Micro-MgB2 has a much more porous structure with corresponding density of 1.0 g/cm3. This indicates that the Mg raw particle size, besides the sintering temperature, is a crucial factor for the formation of high density MgB2 sample, even at the temperature much lower than that of the Mg melting, 650 C. The X-ray diffraction (XRD) pattern shows a good MgB2 phase with small amount of MgO and Mg and the transition temperature, TC, of the Nano-MgB2 was determined as 39 K by the temperature dependent magnetization measurement (M-T), indicating the existence of a good superconducting property.",0406398v1 2004-08-27,Spin reorientation and in-plane magnetoresistance of lightly doped La_{2-x}Sr_{x}CuO_{4} in magnetic fields up to 55 T,"The magnetoresistance (MR) in the in-plane resistivity is measured in magnetic fields up to 55 T in lightly doped La_{2-x}Sr_{x}CuO_{4} in the N\'eel state (x = 0.01) and in the spin-glass state (x = 0.03) using high-quality untwinned single crystals. In both cases, a large negative MR is observed to appear when the magnetic order is established. For x = 0.01, it is found that the MR is indicative of a one-step transition into a high-field weak-ferromagnetic state at around 20 T when the magnetic field is applied from the spin easy axis (b axis), which means that there is no spin-flop transition in the N\'eel state of this material; this is contrary to a previous report, but is natural in light of the peculiar in-plane magnetic susceptibility anisotropy recently found in this system. In the spin-glass state, we observe that the large (up to \sim20%) negative MR saturates at around 40 T, and this MR is found to be essentially isotropic when the magnetic field is rotated within the ab plane. Our data show that the large negative MR is inherent to LSCO in a magnetically ordered state, in which the weak-ferromagnetic (WF) moment becomes well-defined; we discuss that the observed MR is essentially due to the reorientation of the WF moments towards the magnetic field direction both in the N\'eel state and in the spin-glass state.",0408604v1 2005-06-27,Strong-coupling theory of high-temperature superconductivity and colossal magnetoresistance,"We argue that the extension of the BCS theory to the strong-coupling regime describes the high-temperature superconductivity of cuprates and the colossal magnetoresistance (CMR) of ferromagnetic oxides if the phonon dressing of carriers and strong attractive correlations are taken into account. The long-range Froehlich electron-phonon interaction has been identified as the most essential in cuprates providing ""superlight"" lattice polarons and bipolarons. Here some kinetic, magnetic, and more recent thermomagnetic normal state measurements are interpreted in the framework of the strong-coupling theory, including the Nernst effect and normal state diamagnetism. Remarkably, a similar strong-coupling approach offers a simple explanation of CMR in ferromagnetic oxides. The pairing of oxygen holes into heavy bipolarons in the paramagnetic phase and their magnetic pair-breaking in the ferromagnetic phase account for the first-order ferromagnetic phase transition, CMR, isotope effects, and pseudogaps in doped manganites. Here we propose an explanation of the phase coexistence and describe the shape of resistivity of manganites near the transition in the framework of the strong-coupling approach.",0506706v3 2006-06-05,Phenomenological theory of current driven exchange switching in ferromagnetic nanojunctions,"Phenomenological approach is developed in the theory of spin-valve type ferromagnetic junctions to describe exchange switching by current flowing perpendicular to interfaces. Forward and backward current switching effects are described and they may be principally different in nature. Mobile electron spins are considered as being free in all the contacting ferromagnetic layers. Joint action of the following two current effects is investigated: the nonequilibrium longitudinal spin-injection effective field and the transverse spin-transfer surface torque. Dispersion relation for fluctuations is derived and solved for a junction model having spatially localized spin transfer torque: depth of the torque penetration into the free layer is assumed much smaller than the total free layer thickness. Some critical value of the well known Gilbert damping constant is established for the first time. Spin transfer torque dominates in the instability threshold determination for small enough damping constants, while the spin-injection effective field dominates for high damping. Fine interplay between spin transfer torque and spin injection is necessary to provide a hysteretic behavior of the resistance versus current dependence. The state diagram building up shows the possibility of non-stationary (time dependent) nonlinear states arising due to instability development. Calculations lead to the instability rise time values of the order of 0.1 ns. Spin wave resonance frequency spectrum softening occurs under the current growing to the instability threshold. Magnetization fluctuations above the threshold rise oscillating with time for low damping, but rise aperiodically and much more rapid for high damping.",0606102v2 2007-02-28,A local field emission study of partially aligned carbon-nanotubes by AFM probe,"We report on the application of Atomic Force Microscopy (AFM) for studying the Field Emission (FE) properties of a dense array of long and vertically quasi-aligned multi-walled carbon nanotubes grown by catalytic Chemical Vapor Deposition on a silicon substrate. The use of nanometric probes enables local field emission measurements allowing investigation of effects non detectable with a conventional parallel plate setup, where the emission current is averaged on a large sample area. The micrometric inter-electrode distance let achieve high electric fields with a modest voltage source. Those features allowed us to characterize field emission for macroscopic electric fields up to 250 V/$\mu$m and attain current densities larger than 10$^5$ A/cm$^2$. FE behaviour is analyzed in the framework of the Fowler-Nordheim theory. A field enhancement factor $\gamma \approx$ 40-50 and a turn-on field $E_{turn-on} \sim$15 V/$\mu$m at an inter-electrode distance of 1 $\mu$m are estimated. Current saturation observed at high voltages in the I-V characteristics is explained in terms of a series resistance of the order of M$\Omega$. Additional effects as electrical conditioning, CNT degradation, response to laser irradiation and time stability are investigated and discussed.",0702682v1 2007-11-09,Defect healing at room temperature in pentacene thin films and improved transistor performance,"We report on a healing of defects at room temperature in the organic semiconductor pentacene. This peculiar effect is a direct consequence of the weak intermolecular interaction which is characteristic of organic semiconductors. Pentacene thin-film transistors were fabricated and characterized by in situ gated four-terminal measurements. Under high vacuum conditions (base pressure of order 10E-8 mbar), the device performance is found to improve with time. The effective field-effect mobility increases by as much as a factor of two and mobilities up to 0.45 cm2/Vs were achieved. In addition, the contact resistance decreases by more than an order of magnitude and there is a significant reduction in current hysteresis. Oxygen/nitrogen exposure and annealing experiments show the improvement of the electronic parameters to be driven by a thermally promoted process and not by chemical doping. In order to extract the spectral density of trap states from the transistor characteristics, we have implemented a powerful scheme which allows for a calculation of the trap densities with high accuracy in a straightforward fashion. We show the performance improvement to be due to a reduction in the density of shallow traps <0.15 eV from the valence band edge, while the energetically deeper traps are essentially unaffected. This work contributes to an understanding of the shallow traps in organic semiconductors and identifies structural point defects within the grains of the polycrystalline thin films as a major cause.",0711.1457v1 2008-04-05,Strain rate effects in the mechanical response of polymer anchored carbon nanotube foams,"Super-compressible foam-like carbon nanotube films have been reported to exhibit highly nonlinear viscoelastic behaviour in compression similar to soft tissue. Their unique combination of light weight and exceptional electrical, thermal and mechanical properties have helped identify them as viable building blocks for more complex nanosystems and as stand-alone structures for a variety of different applications. In the as-grown state, their mechanical performance is limited by the weak adhesion between the tubes, controlled by the van der Waals forces, and the substrate allowing the forests to split easily and to have low resistance in shear. Under axial compression loading carbon nanotubes have demonstrated bending, buckling8 and fracture9 (or a combination of the above) depending on the loading conditions and on the number of loading cycles. In this work, we partially anchor dense vertically aligned foam-like forests of carbon nanotubes on a thin, flexible polymer layer to provide structural stability, and report the mechanical response of such systems as a function of the strain rate. We test the sample under quasi-static indentation loading and under impact loading and report a variable nonlinear response and different elastic recovery with varying strain rates. A Bauschinger-like effect is observed at very low strain rates while buckling and the formation of permanent defects in the tube structure is reported at very high strain rates. Using high-resolution transmission microscopy",0804.0868v1 2008-04-10,Electrical transport and ferromagnetism in Ga1-xMnxAs synthesized by ion implantation and pulsed-laser melting,"We present a detailed investigation of the magnetic and magnetotransport properties of thin films of ferromagnetic Ga1-xMnxAs synthesized using ion implantation and pulsed-laser melting (II-PLM). The field and temperature-dependent magnetization, magnetic anisotropy, temperature-dependent resistivity, magnetoresistance, and Hall effect of II-PLM Ga1-xMnxAs films have all of the characteristic signatures of the strong p-d interaction of holes and Mn ions observed in the dilute hole-mediated ferromagnetic phase. The ferromagnetic and electrical transport properties of II-PLM films correspond to the peak substitutional Mn concentration meaning that the non-uniform Mn depth distribution is unimportant in determining the film properties. Good quantitative agreement is found with films grown by low temperature molecular beam epitaxy (LT-MBE) and having the similar substitutional Mn_Ga composition. Additionally, we demonstrate that II-PLM Ga1-xMnxAs films are free from interstitial Mn_I because of the high temperature processing. At high Mn implantation doses the kinetics of solute redistribution during solidification alone determine the maximum resulting Mn_Ga concentration. Uniaxial anisotropy between in-plane [-110]and [110] directions is present in II-PLM Ga1-xMnxAs giving evidence for this being an intrinsic property of the carrier-mediated ferromagnetic phase.",0804.1612v1 2010-01-26,Signature of checkerboard fluctuations in the phonon spectra of a possible polaronic metal La1.2Sr1.8Mn2O7,"Charge carriers in low-doped semiconductors may distort the atomic lattice and trap themselves forming so-called small polarons. High carrier concentrations can lead to short range ordered polarons (large polarons) and even to long range charge and orbital order. Both systems should be insulating with a large electrical resistivity, which decreases with increasing temperature. However, photoemission measurements recently found a polaronic pseudogap, in a metallic phase of La2-2xSr1+2xMn2O7. This layered manganite is famous for colossal magnetoresistance (CMR) associated with a phase transition from this low-temperature metallic phase to a high temperature insulating phase. Broad charge order peaks due to large polarons observed by neutron and x-ray scattering in the insulating phase disappear when La2-2xSr1+2xMn2O7 becomes metallic. We report results of inelastic neutron scattering measurements showing that polarons remain inside the metallic phase as fluctuations that strongly broaden and soften certain phonons near the wave vectors where the charge order peaks appeared in the insulating phase. Our findings imply that polaronic signatures in metals may generally come from a competing insulating charge-ordered phase. It is highly relevant to cuprate superconductors with both a pseudogap, and a similar phonon effect associated with a competing stripe order.",1001.4636v1 2010-04-28,"Synthesis, Structure and Properties of Tetragonal Sr2M3As2O2 (M3 = Mn3, Mn2Cu and MnZn2) Compounds Containing Alternating CuO2-Type and FeAs-Type Layers","Polycrystalline samples of Sr2Mn2CuAs2O2, Sr2Mn3As2O2, and Sr2Zn2MnAs2O2 were synthesized. Their temperature- and applied magnetic field-dependent structural, transport, thermal, and magnetic properties were characterized by means of x-ray and neutron diffraction, electrical resistivity rho, heat capacity, magnetization and magnetic susceptibility measurements. These compounds have a body-centered-tetragonal crystal structure (space group I4/mmm) that consists of MO2 (M = Zn and/or Mn) oxide layers similar to the CuO2 layers in high superconducting transition temperature Tc cuprate superconductors, and intermetallic MAs (M = Cu and/or Mn) layers similar to the FeAs layers in high-Tc pnictides. These two types of layers alternate along the crystallographic c-axis and are separated by Sr atoms. The site occupancies of Mn, Cu and Zn were studied using Rietveld refinements of x-ray and neutron powder diffraction data. The temperature dependences of rho suggest metallic character for Sr2Mn2CuAs2O2 and semiconducting character for Sr2Mn3As2O2 and Sr2Zn2MnAs2O2. Sr2Mn2CuAs2O2 is inferred to be a ferrimagnet with a Curie temperature TC = 95(1) K. Remarkably, we find that the magnetic ground state structure changes from a G-type antiferromagnetic structure in Sr2Mn3As2O2 to an A-type ferrimagnetic structure in Sr2Mn2CuAs2O2 in which the Mn ions in each layer are ferromagnetically aligned, but are antiferromagnetically aligned between layers.",1004.5038v1 2011-06-21,Transport properties and anisotropy in rare earth doped CaFe2As2 single crystals with Tc above 40 K,"In this paper we report the superconductivity above 40 K in the electron doping single crystal Ca1-xRexFe2As2 (Re = La, Ce, Pr). The x-ray diffraction patterns indicate high crystalline quality and c-axis orientation. the resistivity anomaly in the parent compound CaFe2As2 is completely suppressed by partial replacement of Ca by rare earth and a superconducting transition reaches as high as 43 K, which is higher than the value in electron doping FeAs-122 compounds by substituting Fe ions with transition metal, even surpasses the highest values observed in hole doping systems with a transition temperature up to 38 K. The upper critical field has been determined with the magnetic field along ab-plane and c-axis, yielding the anisotropy of 2~3. Hall-effect measurements indicate that the conduction in this material is dominated by electron like charge carriers. Our results explicitly demonstrate the feasibility of inducing superconductivity in Ca122 compounds via electron doping using aliovalent rare earth substitution into the alkaline earth site, which should add more ingredients to the underlying physics of the iron-based superconductors.",1106.4208v1 2012-02-13,Graphene-on-Diamond Devices with Enhanced Current-Carrying Capacity: Carbon sp2-on-sp3 Technology,"Graphene demonstrated potential for practical applications owing to its excellent electronic and thermal properties. Typical graphene field-effect transistors and interconnects built on conventional SiO2/Si substrates reveal the breakdown current density on the order of 1 uA/nm2 (i.e. 10^8 A/cm2) which is ~100\times larger than the fundamental limit for the metals but still smaller than the maximum achieved in carbon nanotubes. We show that by replacing SiO2 with synthetic diamond one can substantially increase the current-carrying capacity of graphene to as high as ~18 uA/nm2 even at ambient conditions. Our results indicate that graphene's current-induced breakdown is thermally activated. We also found that the current carrying capacity of graphene can be improved not only on the single-crystal diamond substrates but also on an inexpensive ultrananocrystalline diamond, which can be produced in a process compatible with a conventional Si technology. The latter was attributed to the decreased thermal resistance of the ultrananocrystalline diamond layer at elevated temperatures. The obtained results are important for graphene's applications in high-frequency transistors, interconnects, transparent electrodes and can lead to the new planar sp2-on-sp3 carbon-on-carbon technology.",1202.2886v1 2012-07-12,Structure and electronic transport in graphene wrinkles,"Wrinkling is a ubiquitous phenomenon in two-dimensional membranes. In particular, in the large-scale growth of graphene on metallic substrates, high densities of wrinkles are commonly observed. Despite their prevalence and potential impact on large-scale graphene electronics, relatively little is known about their structural morphology and electronic properties. Surveying the graphene landscape using atomic force microscopy, we found that wrinkles reach a certain maximum height before folding over. Calculations of the energetics explain the morphological transition, and indicate that the tall ripples are collapsed into narrow standing wrinkles by van der Waals forces, analogous to large-diameter nanotubes. Quantum transport calculations show that conductance through these collapsed wrinkle structures is limited mainly by a density-of-states bottleneck and by interlayer tunneling across the collapsed bilayer region. Also through systematic measurements across large numbers of devices with wide folded wrinkles, we find a distinct anisotropy in their electrical resistivity, consistent with our transport simulations. These results highlight the coupling between morphology and electronic properties, which has important practical implications for large-scale high-speed graphene electronics.",1207.2994v1 2012-09-06,Terahertz time-domain spectroscopic ellipsometry: Instrumentation and calibration,"We present a new instrumentation and calibration procedure for terahertz time-domain spectroscopic ellipsometry (THz-TDSE) that is a newly established characterization technique. The experimental setup is capable of providing arbitrary angle of incidence in the range of $15^\circ$--$85^\circ$ in the reflection geometry, and with no need for realignment. The setup is also configurable easily into transmission geometry. For this setup, we successfully used hollow core photonic band gap fiber with no pre-chirping in order to deliver a femtosecond laser into a THz photoconductive antenna detector, which is the first demonstration of this kind. The proposed calibration scheme can compensate for the non-ideality of the polarization response of the THz photoconductive antenna detector as well as that of wire grid polarizers used in the setup. In the calibration scheme, the ellipsometric parameters are obtained through a regression algorithm which we have adapted from the conventional regression calibration method developed for rotating element optical ellipsometers, and used here for the first time for THz-TDSE. As a proof-of-principle demonstration, results are presented for a high resistivity silicon substrate as well as an opaque Si substrate with a high phosphorus concentration. We also demonstrate the capacity to measure a few micron thick grown thermal oxide on top of Si. Each sample was characterized by THz-TDSE in reflection geometry with different angle of incidence.",1209.1294v2 2013-05-09,Fermilab experience of post-annealing losses in SRF niobium cavities due to furnace contamination and the ways to its mitigation: a pathway to processing simplification and quality factor improvement,"We investigate the effect of high temperature treatments followed by only high-pressure water rinse (HPR) of superconducting radio frequency (SRF) niobium cavities. The objective is to provide a cost effective alternative to the typical cavity processing sequence, by eliminating the material removal step post furnace treatment while preserving or improving the RF performance. The studies have been conducted in the temperature range 800-1000C for different conditions of the starting substrate: large grain and fine grain, electro-polished (EP) and centrifugal barrel polished (CBP) to mirror finish. An interesting effect of the grain size on the performances is found. Cavity results and samples characterization show that furnace contaminants cause poor cavity performance, and a practical solution is found to prevent surface contamination. Extraordinary values of residual resistances ~ 1 nOhm and below are then consistently achieved for the contamination-free cavities. These results lead to a more cost-effective processing and improved RF performance, and, in conjunction with CBP, open a potential pathway to acid-free processing.",1305.2182v2 2013-06-03,Electrical switching dynamics and broadband microwave characteristics of VO2 RF devices,"Vanadium dioxide is a correlated electron system that features a metal-insulator phase transition (MIT) above room temperature and is of interest in high speed switching devices. Here, we integrate VO2 into two-terminal coplanar waveguides and demonstrate a large resistance modulation of the same magnitude (>10^3) in both electrically (i.e. by bias voltage, referred to as E-MIT) and thermally (T-MIT) driven transitions. We examine transient switching characteristics of the E-MIT and observe two distinguishable time scales for switching. We find an abrupt jump in conductivity with a rise time of the order of 10 ns followed by an oscillatory damping to steady state on the order of several {\mu}s. We characterize the RF power response in the On state and find that high RF input power drives VO2 further into the metallic phase, indicating that electromagnetic radiation-switching of the phase transition may be possible. We measure S-parameter RF properties up to 13.5 GHz. Insertion loss is markedly flat at 2.95 dB across the frequency range in the On state and sufficient isolation of over 25 dB is observed in the Off state. We are able to simulate the RF response accurately using both lumped element and 3D electromagnetic models. Extrapolation of our results suggests that optimizing device geometry can reduce insertion loss further and maintain broadband flatness up to 40 GHz.",1306.0292v1 2013-07-16,ZnS/Diamond Composite Coatings for Infrared Transmission Applications Formed by the Aerosol Deposition Method,"The deposition of nano-crystalline ZnS/diamond composite protective coatings on silicon, sapphire, and ZnS substrates, as a preliminary step to coating infrared transparent ZnS substrates from powder mixtures by the aerosol deposition method is presented. Advantages of the aerosol deposition method include the ability to form dense, nanocrystalline films up to hundreds of microns thick at room temperature and at a high deposition rate on a variety of substrates. Deposition is achieved by creating a pressure gradient that accelerates micrometer-scale particles in an aerosol to high velocity. Upon impact with the target substrate the particles fracture and embed. Continued deposition forms the thick compacted film. Deposition from an aerosolized mixture of ZnS and diamond powders onto all targets results in linear trend from apparent sputter erosion of the substrate at 100% diamond to formation of a film with increasing fractions of ZnS. The crossover from abrasion to film formation on sapphire occurs above about 50% ZnS and a mixture of 90% ZnS and 10% diamond forms a well-adhered film of about 0.7 \mu m thickness at a rate of 0.14 \mu m/min. Resulting films are characterized by scanning electron microscopy, profilometry, infrared transmission spectroscopy, and x-ray photoemission spectroscopy. These initial films mark progress toward the future goal of coating ZnS substrates for abrasion resistance.",1307.4319v1 2013-10-01,Unexpected Giant Superconducting Fluctuation and Anomalous Semiconducting Normal State in NdO1-xFxBi1-yS2 Single Crystals,"The BiS2-based superconductors were discovered recently. The superconductivity has been proved by many other groups. Since the previous experiments were all done on polycrystalline samples, therefore there remains a concern whether the superconductivity is really derived from the materials intrinsically or from some secondary phases. Experiments on single crystals are highly desired. In this paper, we report the successful growth of the NdO1-xFxBi1-yS2 single crystals. Resistive and magnetic measurements reveal that the bulk superconducting transition occurs at about 5 K, while an unexpected giant superconducting fluctuation appears at temperatures as high as 2-4 kBTC. Analysis based on the anisotropic Ginzbaug-Landau theory gives an anisotropy of 30-45. Two gap features with magnitudes of about 3.5+-0.3 meV and 7.5+-1 meV were observed by scanning tunneling spectroscopy. The smaller gap is associated with the bulk superconducting transition at about 5 K yielding a huge ratio 2Delta_s/kBTc =16.8, the larger gap remains up to about 26 K. The normal state recovered by applying a high magnetic field shows an anomalous semiconducting behavior. All these suggest that the superconductivity in this newly discovered superconductor cannot be formatted into the BCS theory.",1310.0377v1 2014-06-26,Electron localization and possible phase separation in the absence of a charge density wave in single-phase 1T-VS$_2$,"We report on a systematic study of the structural, magnetic and transport properties of high-purity 1T-VS$_2$ powder samples prepared under high pressure. The results differ notably from those previously obtained by de-intercalating Li from LiVS$_2$. First, no Charge Density Wave (CDW) is found by transmission electron microscopy down to 94 K. Though, \textit{ab initio} phonon calculations unveil a latent CDW instability driven by an acoustic phonon softening at the wave vector ${\bf q}_{CDW} \approx$ (0.21,0.21,0) previously reported in de-intercalated samples. A further indication of latent lattice instability is given by an anomalous expansion of the V-S bond distance at low temperature. Second, infrared optical absorption and electrical resistivity measurements give evidence of non metallic properties, consistent with the observation of no CDW phase. On the other hand, magnetic susceptibility and NMR data suggest the coexistence of localized moments with metallic carriers, in agreement with \textit{ab initio} band structure calculations. This discrepancy is reconciled by a picture of electron localization induced by disorder or electronic correlations leading to a phase separation of metallic and non-metallic domains in the nm scale. We conclude that 1T-VS$_2$ is at the verge of a CDW transition and suggest that residual electronic doping in Li de-intercalated samples stabilizes a uniform CDW phase with metallic properties.",1406.6945v1 2014-11-07,Upgrade of the ALICE Inner Tracking System,"During the Long Shutdown 2 of the LHC in 2018/2019, the ALICE experiment plans the installation of a novel Inner Tracking System. It will replace the current six layer detector system with a seven layer detector using Monolithic Active Pixel Sensors. The upgraded Inner Tracking System will have significantly improved tracking and vertexing capabilities, as well as readout rate to cope with the expected increased Pb-Pb luminosity of the LHC. The choice of Monolithic Active Pixel Sensors has been driven by the specific requirements of ALICE as a heavy ion experiment dealing with rare processes at low transverse momenta. This leads to stringent requirements on the material budget of 0.3$% X/X_{0}$ per layer for the three innermost layers. Furthermore, the detector will see large hit densities of $\sim 19 \mathrm{cm}^{-2}/\mathrm{event}$ on average for minimum-bias events in the inner most layer and has to stand moderate radiation loads of 700 kRad TID and $1\times 10^{13}$ 1 MeV n$_\mathrm{eq}/\mathrm{cm}^{2}$ NIEL at maximum. The Monolithic Active Pixel Sensor detectors are manufactured using the TowerJazz 0.18 $\mu$m CMOS Imaging Sensor process on wafers with a high-resistivity epitaxial layer. This contribution summarises the recent R&D activities and focuses on results on the large-scale pixel sensor prototypes.",1411.1802v2 2014-12-26,High Pressure Induced Binding Between Linear Carbon Chains and Nanotubes,"Recent studies of single-walled carbon nanotubes (CNTs) in aqueous media have showed that water can significantly affect the tube mechanical properties. CNTs under hydrostatic compression can preserve their elastic properties up to large pressure values, while exhibiting exceptional resistance to mechanical loadings. It was experimentally observed that CNTs with encapsulated linear carbon chains (LCCs), when subjected to high hydrostatic pressure values, present irreversible red shifts in some of their vibrational frequencies. In order to address the cause of this phenomenon, we have carried out fully atomistic reactive (ReaxFF) molecular dynamics (MD) simulations for model structures mimicking the experimental conditions. We have considered the cases of finite and infinite (cyclic boundary conditions) CNTs filled with LCCs (LCC inside CNTs) of different lengths (from 9 up to 40 atoms). Our results show that increasing the hydrostatic pressure causes the CNT to be deformed in an inhomogeneous way due to the LCC presence. The LCC-CNT interface regions exhibit convex curvatures, which results in more reactive sites, thus favoring the formation of covalent chemical bonds between the chain and the nanotube. This process is irreversible with the newly formed bonds continuing to exist even after releasing the external pressure and causing an irreversibly red shift in the chain vibrational modes from 1850 to 1500 cm$^{-1}$.",1412.7966v1 2015-01-29,Superconducting properties of sulfur-doped iron selenide,"The recent discovery of high-temperature superconductivity in single-layer iron selenide has generated significant experimental interest for optimizing the superconducting properties of iron-based superconductors through the lattice modification. For simulating the similar effect by changing the chemical composition due to S doping, we investigate the superconducting properties of high-quality single crystals of FeSe$_{1-x}$S$_{x}$ ($x$=0, 0.04, 0.09, and 0.11) using magnetization, resistivity, the London penetration depth, and low temperature specific heat measurements. We show that the introduction of S to FeSe enhances the superconducting transition temperature $T_{c}$, anisotropy, upper critical field $H_{c2}$, and critical current density $J_{c}$. The upper critical field $H_{c2}(T)$ and its anisotropy are strongly temperature dependent, indicating a multiband superconductivity in this system. Through the measurements and analysis of the London penetration depth $\lambda _{ab}(T)$ and specific heat, we show clear evidence for strong coupling two-gap $s$-wave superconductivity. The temperature-dependence of $\lambda _{ab}(T)$ calculated from the lower critical field and electronic specific heat can be well described by using a two-band model with $s$-wave-like gaps. We find that a $d$-wave and single-gap BCS theory under the weak-coupling approach can not describe our experiments. The change of specific heat induced by the magnetic field can be understood only in terms of multiband superconductivity.",1501.07346v1 2015-09-28,"Thermoelectric properties of rare earth filled type-I like Clathrate, Dy8Al16Si30","Type-I clathrates with a cage structure are known to be of importance for thermoelectric applications as the cage can be filled with a guest atom which leads to reduced thermal conductivity. Among the type-I clathrates, Si-based alloys are of relevance for high temperature application and most importantly because they are made of earth abundant elements. Dysprosium, Dy has been chosen as the guest atom because of its large mass and small size compared to divalent alkali metal ion. The Dy8Al16Si30, DAS, alloy has been synthesized by arc melting of pure elements followed by annealing at 780 K for 7 days. Structural characterization performed using XRD and SEM indicates presence of both binary and ternary silicides, DySi2, DyAl2Si2 together with Al solid solution and Si. The phase mixture remains unchanged even after annealing. The microstructure has a typical dendritic structure with interdendritic phases, signifying a slow, liquid transformation after arc melting. The Seebeck coefficient is found to be positive, a p-type and increases with increasing temperature both before and after annealing. The resistivity is found to be low in the whole temperature range, 2 to 10 micro Ohm m and increases with increasing temperature. The power factor in the as-prepared state is found to be higher at all temperatures in the range 300 K to 700 K compared to annealed state. The thermal conductivity however has been found to decrease on annealing from an unusually high value of 100 W/m K to 50 W/m K.",1509.08277v1 2016-01-06,Observation of quantum Hall plateau-plateau transition and scaling behavior of the zeroth Landau level in graphene p-n-p junctions,"We report distinctive magnetotransport properties of a graphene p-n-p junction prepared by controlled diffusion of metallic contacts. In most cases, materials deposited on a graphene surface introduce substantial carrier scattering, which greatly reduces the high mobility of intrinsic graphene. However, we show that an oxide layer only weakly perturbs the carrier transport, which enables fabrication of a high-quality graphene p-n-p junction through a one-step and resist-free method. The measured conductance-gate voltage $(G-V_G)$ curves can be well described by a metal contact model, which confirms the charge density depinning due to the oxide layer. The graphene p-n-p junction samples exhibit pronounced quantum Hall effect, a well-defined transition point of the zeroth Landau level (LL), and scaling behavior. The scaling exponent obtained from the evolution of the zeroth LL width as a function of temperature exhibits a relatively low value of $\kappa=0.21\pm0.01$. Moreover, we calculate the energy level for the LLs based on the distribution of plateau-plateau transition points, further validating the assignment of the LL index of the QH plateau-plateau transition.",1601.01155v1 2017-02-07,Resonant spin transfer torque nano-oscillators,"Spin transfer torque nano-oscillators are potential candidates for replacing the traditional inductor based voltage controlled oscillators in modern communication devices. Typical oscillator designs are based on trilayer magnetic tunnel junctions which are disadvantaged by low power outputs and poor conversion efficiencies. In this letter, we theoretically propose to use resonant spin filtering in pentalayer magnetic tunnel junctions as a possible route to alleviate these issues and present device designs geared toward a high microwave output power and an efficient conversion of the d.c. input power. We attribute these robust qualities to the resulting non-trivial spin current profiles and the ultra high tunnel magnetoresistance, both arising from resonant spin filtering. The device designs are based on the nonequilibrium Green's function spin transport formalism self-consistently coupled with the stochastic Landau-Lifshitz-Gilbert-Slonczewski's equation and the Poisson's equation. We demonstrate that the proposed structures facilitate oscillator designs featuring a large enhancement in microwave power of around $775\%$ and an efficiency enhancement of over $1300\%$ in comparison with typical trilayer designs. We also rationalize the optimum operating regions via an analysis of the dynamic and static device resistances. This work sets stage for pentalyer spin transfer torque nano-oscillator device designs that extenuate most of the issues faced by the typical trilayer designs.",1702.01869v1 2017-02-18,Ultralow 1/f Noise in a Heterostructure of Superconducting Epitaxial Cobalt-Disilicide Thin Film on Silicon,"High-precision resistance noise measurements indicate that the epitaxial CoSi$_2$/Si hetero-structures at 150 K and 2 K (slightly above its superconducting transition temperature $T_c$ of 1.54 K) exhibit an unusually low 1/f noise level in the frequency range of 0.008-0.2 Hz. This corresponds to an upper limit of Hooge constant $\gamma \leq 3 \times 10^{-6}$, about 100 times lower than that of single-crystalline aluminum films on SiO$_2$ capped Si substrates. Supported by high-resolution cross-sectional transmission electron microscopy studies, our analysis reveals that the 1/f noise is dominated by excess interfacial Si atoms and their dimer reconstruction induced fluctuators. Unbonded orbitals (i.e., dangling bonds) on excess Si atoms are intrinsically rare at the epitaxial CoSi$_2$/Si(100) interface, giving limited trapping-detrapping centers for localized charges. With its excellent normal-state properties, CoSi$_2$ has been used in silicon-based integrated circuits for decades. The intrinsically low noise properties discovered in this work could be utilized for developing quiet qubits and scalable superconducting circuits for future quantum computing.",1702.05566v1 2017-06-03,Electronic in-plane symmetry breaking at field-tuned quantum criticality in CeRhIn5,"Electronic nematics are exotic states of matter where electronic interactions break a rotational symmetry of the underlying lattice, in analogy to the directional alignment without translational order in nematic liquid crystals. Intriguingly such phases appear in the copper- and iron-based superconductors, and their role in establishing high-temperature superconductivity remains an open question. Nematicity may take an active part, cooperating or competing with superconductivity, or may appear accidentally in such systems. Here we present experimental evidence for a phase of nematic character in the heavy fermion superconductor CeRhIn5. We observe a field-induced breaking of the electronic tetragonal symmetry of in the vicinity of an antiferromagnetic (AFM) quantum phase transition at Hc~50T. This phase appears in out-of-plane fields of H*~28T and is characterized by substantial in-plane resistivity anisotropy. The anisotropy can be aligned by a small in-plane field component, with no apparent connection to the underlying crystal structure. Furthermore no anomalies are observed in the magnetic torque, suggesting the absence of metamagnetic transitions in this field range. These observations are indicative of an electronic nematic character of the high field state in CeRhIn5. The appearance of nematic behavior in a phenotypical heavy fermion superconductor highlights the interrelation of nematicity and unconventional superconductivity, suggesting nematicity to be a commonality in such materials.",1706.00963v1 2017-09-03,Giant tunnel magnetoresistance with a single magnetic phase-transition electrode,"Magnetic phase transition tunnel magnetoresistance (MPT-TMR) effect with a single magnetic electrode has been investigated by first-principles calculations. The calculations show that the MPT-TMR of FeRh/MgO/Cu tunnel junction can be as high as hundreds of percent when the magnetic structure of FeRh changes from G-type antiferromagnetic (GAFM) to ferromagnetic order. This new type of MPT-TMR may be superior to the tunnel anisotropic magnetoresistance because of its huge magneto-resistance effect and similar structural simplicity. The main mechanism for the giant MPT-TMR can be attributed to the formation of interface resonant states at GAFM-FeRh/MgO interface. A direct FeRh/MgO interface is found to be necessary for achieving high MPT-TMR experimentally. Moreover, we find the FeRh/MgO interface with FeRh in ferromagnetic phase has nearly full spin-polarization due to the negligible majority transmission and significantly different Fermi surface of two spin channels. Thus, it may act as a highly efficient and tunable spin-injector. In addition, electric field driven MPT of FeRh-based hetero-magnetic nanostructures can be utilized to design various energy efficient tunnel junction structures and the corresponding lower power consumption devices. Our results will stimulate further experimental investigations of MPT-TMR and other fascinating phenomenon of FeRh-based tunnel junctions that may be promising in antiferromagnetic spintronics.",1709.00687v2 2017-11-08,"X-ray photoelectron spectroscopy, Magnetotransport and Magnetization study of Nb2PdS5 superconductor","In the present report, we investigate various properties of the Nb2PdS5 superconductor. Scanning electron microscopy displayed slabs like laminar growth of Nb2PdS5while X-ray photoelectron spectroscopy exhibited the hybridization of Sulphur (2p) with both Palladium (3d)and Niobium (3d). High field (140kOe) magneto-transport measurements revealed that superconductivity (Tc onset =7K and Tc R = 0 = 6.2K) of the studied Nb2PdS5material is quite robust against magnetic field with the upper critical field (Hc2) outside the Pauli paramagnetic limit. Thermally activated flux flow (TAFF) of the compound showed that resistivity curves follow Arrhenius behaviour. The activation energy for Nb2PdS5 is found to decrease from 15.15meV at 10kOe to 2.35meV at 140kOe. Seemingly, the single vortex pinning is dominant in low field regions, while collective pinning is dominant in high field region. The temperature dependence of AC susceptibility confirmed the Tc at 6K, further varying amplitude and frequency showed well coupled granular nature of superconductivity. The lower critical field (Hc1) is extracted from DC magnetisation measurements at various T below Tc. It is found that Hc1(T) of Nb2PdS5 material seemingly follows the multiband nature of superconductivity.",1711.02830v1 2017-11-10,Thermodynamic Studies of \b{eta}-Ga2O3 Nanomembrane Field-Effect Transistors on a Sapphire Substrate,"The self-heating effect is a severe issue for high-power semiconductor devices, which degrades the electron mobility and saturation velocity, and also affects the device reliability. On applying an ultrafast and high-resolution thermoreflectance imaging technique, the direct self-heating effect and surface temperature increase phenomenon are observed on novel top-gate \b{eta}-Ga2O3 on insulator field-effect transistors. Here, we demonstrate that by utilizing a higher thermal conductivity sapphire substrate rather than a SiO2/Si substrate, the temperature rise above room temperature of \b{eta}-Ga2O3 on the insulator field-effect transistor can be reduced by a factor of 3 and thereby the self-heating effect is significantly reduced. Both thermoreflectance characterization and simulation verify that the thermal resistance on the sapphire substrate is less than 1/3 of that on the SiO2/Si substrate. Therefore, maximum drain current density of 535 mA/mm is achieved on the sapphire substrate, which is 70% higher than that on the SiO2/Si substrate due to reduced self-heating. Integration of \b{eta}-Ga2O3 channel on a higher thermal conductivity substrate opens a new route to address the low thermal conductivity issue of \b{eta}-Ga2O3 for power electronics applications.",1711.03672v1 2018-03-28,Study of nitrogen ion doping of titanium dioxide films,"This study reports on the properties of nitrogen doped titanium dioxide $TiO_2$ thin films considering the application as transparent conducting oxide (TCO). Sets of thin films were prepared by sputtering a titanium target under oxygen atmosphere on a quartz substrate at 400 or 500{\deg}C. Films were then doped at the same temperature by 150 eV nitrogen ions. The films were prepared in Anatase phase which was maintained after doping. Up to 30at% nitrogen concentration was obtained at the surface, as determined by in situ x-ray photoelectron spectroscopy (XPS). Such high nitrogen concentration at the surface lead to nitrogen diffusion into the bulk which reached about 25 nm. Hall measurements indicate that average carrier density reached over $10^{19} cm^{-3}$ with mobility in the range of $0.1$ to $1 cm^2V^{-1}s^{-1}$. Resistivity about $3.10^{-1} \Omega cm$ could be obtained with 85% light transmission at 550 nm. These results indicate that low energy implantation is an effective technique for $TiO_2$ doping that allows an accurate control of the doping process independently from the TiO2 preparation. Moreover, this doping route seems promising to attain high doping levels without significantly affecting the film structure. Such approach could be relevant for preparation of $N:TiO_2$ transparent conduction electrodes (TCE).",1803.10828v1 2018-06-15,Quantum anomalous Hall multilayers grown by molecular beam epitaxy,"Quantum anomalous Hall (QAH) effect is a quantum Hall effect that occurs without the need of external magnetic field. A system composed of multiple parallel QAH layers is an effective high Chern number QAH insulator and the key to the applications of the dissipationless chiral edge channels in low energy consumption electronics. Such a QAH multilayer can also be engineered into other exotic topological phases such as a magnetic Weyl semimetal with only one pair of Weyl points. This work reports the first experimental realization of QAH multilayers in the superlattices composed of magnetically doped (Bi,Sb)$_2$Te$_3$ topological insulator and CdSe normal insulator layers grown by molecular beam epitaxy. The obtained multilayer samples show quantized Hall resistance $h/Ne$$^2$, where $h$ is the Planck's constant, $e$ is the elementary charge and $N$ is the number of the magnetic topological insulator layers, resembling a high Chern number QAH insulator.",1806.05923v1 2018-09-26,Rare earth permanent magnets prepared by hot deformation process,"Hot deformation process is one of the primary methods to produce anisotropic rare earth permanent magnets. Firstly, rapidly quenched powder flakes with nanocrystal structure are condensed into the full dense isotropic precursors by hot pressing process. And then, the prepared isotropic precursors are hot deformed to produce high-anisotropy uniaxial bulk rare earth permanent magnets, in which the highly textured structure is obtained in the hot plastic deformation process. The obtained hot-deformed magnets possess many advantages, such as near net-shape, outstanding corrosion resistance and ultrafine-grain structure. The noteworthy effects of preparation parameters employed in hot-pressing and deformation processes on the magnetic properties and microstructures characterizations are systemically summarized in this academic monograph. As a near net-shape technique, hot deformation process has noteworthy advantages in producing irregular shape magnets, especially for radially oriented ring-shape magnets with high length-diameter ratio or thin wall. The difficulties in producing crack-free, homogeneous and non-decentered ring-shaped magnets are basically resolved through mold design, adjustment of deformation parameters and application of theoretical simulation. Considering the characteristics of hot-deformed magnets, such as the grain shapes and sizes, anisotropic distribution of intergranular phases, etc., there is practical significance to study and improve the mechanical, electric properties and thermal stability to enlarge the applicable area of hot-deformed magnets or ring-shaped magnets.",1809.09838v1 2018-11-05,SkyLogic - A proposal for a skyrmion logic device,"This work proposes a novel logic device (SkyLogic) based on skyrmions, which are magnetic vortex-like structures that have low depinning current density and are robust to defects. A charge current sent through a polarizer ferromagnet (P-FM) nucleates a skyrmion at the input end of an intra-gate FM interconnect with perpendicular magnetic anisotropy (PMA-FM). The output end of the PMA--FM forms the free layer of an MTJ stack. A spin Hall metal (SHM) is placed beneath the PMA-FM. The skyrmion is propagated to the output end of the PMA-FM by passing a charge current through the SHM. The resistance of the MTJ stack is low (high) when a skyrmion is present (absent) in the free layer, thereby realizing an inverter. A framework is developed to analyze the performance of the SkyLogic device. A circuit-level technique is developed that counters the transverse displacement of skyrmion in the PMA-FM and allows use of high current densities for fast propagation. The design space exploration of the PMA-FM material parameters is performed to obtain an optimal design point. At the optimal point, we obtain an inverter delay of 434 ps with a switching energy of 7.1 fJ.",1811.02016v1 2019-09-06,Electronic correlation determining correlated plasmons in Sb-doped Bi$_2$Se$_3$,"Electronic correlation is believed to play an important role in exotic phenomena such as insulator-metal transition, colossal magneto resistance and high temperature superconductivity in correlated electron systems. Recently, it has been shown that electronic correlation may also be responsible for the formation of unconventional plasmons. Herewith, using a combination of angle-dependent spectroscopic ellipsometry, angle resolved photoemission spectroscopy and Hall measurements all as a function of temperature supported by first-principles calculations, the existence of low-loss high-energy correlated plasmons accompanied by spectral weight transfer, a fingerprint of electronic correlation, in topological insulator (Bi$_{0.8}$Sb$_{0.2}$)$_2$Se$_3$ is revealed. Upon cooling, the density of free charge carriers in the surface states decreases whereas those in the bulk states increase, and that the newly-discovered correlated plasmons are key to explaining this phenomenon. Our result shows the importance of electronic correlation in determining new correlated plasmons and opens a new path in engineering plasmonic-based topologically-insulating devices.",1909.02703v1 2020-03-30,"Growth and transport properties of Mg3X2 (X = Sb, Bi) single crystals","The discovery of high thermoelectric performance in n-type polycrystalline Mg3(Sb,Bi)2 based Zintl compounds has ignited intensive research interest. However, some fundamental questions concerning the anisotropic transport properties and the origin of intrinsically low thermal conductivity are still elusive, requiring the investigation of single crystals. In this work, high-quality p-type Mg3Sb2 and Mg3Bi2 single crystals have been grown by using a self-flux method. The electrical resistivity \r{ho} of Mg3Bi2 single crystal displays an anisotropy with \r{ho} in-plane twice larger than out-of-plane. The low-temperature heat capacity and lattice thermal conductivity of Mg3Sb2 and Mg3Bi2 single crystals have been investigated by using the Debye-Callaway model, from which the existence of low-lying vibration mode could be concluded. Large Gr\""uneisen parameters and strong anharmonicity are found responsible for the intrinsically low thermal conductivity. Moreover, grain boundary scattering does not contribute significantly to suppress the lattice thermal conductivity of polycrystalline Mg3Sb2. Our results provide insights into the intrinsic transport properties of Mg3X2 and could pave a way to realize enhanced thermoelectric performance in single-crystalline Mg3X2-based Zintl compounds.",2003.13313v1 2017-03-13,Extremely high magnetoresistance and conductivity in the type-II Weyl semimetals WP2 and MoP2,"The peculiar band structure of semimetals exhibiting Dirac and Weyl crossings can lead to spectacular electronic properties such as large mobilities accompanied by extremely high magnetoresistance. In particular, two closely neighbouring Weyl points of the same chirality are protected from annihilation by structural distortions or defects, thereby significantly reducing the scattering probability between them. Here we present the electronic properties of the transition metal diphosphides, WP2 and MoP2, that are type-II Weyl semimetals with robust Weyl points. We present transport and angle resolved photoemission spectroscopy measurements, and first principles calculations. Our single crystals of WP2 display an extremely low residual low-temperature resistivity of 3 nohm-cm accompanied by an enormous and highly anisotropic magnetoresistance above 200 million % at 63 T and 2.5 K. These properties are likely a consequence of the novel Weyl fermions expressed in this compound. We observe a large suppression of charge carrier backscattering in WP2 from transport measurements.",1703.04527v3 2017-03-20,Exceptional Anti-Icing Performance of Self-Impregnating Slippery Surfaces,"A heat exchange interface at subzero temperature in a water vapor environment, exhibits high probability of frost formation due to freezing condensation, a factor that markedly decreases the heat transfer efficacy due to the considerable thermal resistance of ice. Here we report a novel strategy to delay ice nucleation on these types of solid-water vapor interfaces. With a process-driven mechanism, a self-generated liquid intervening layer immiscible to water, is deposited on a textured superhydrophobic surface and acts as a barrier between the water vapor and the solid substrate. This liquid layer imparts remarkable slippery conditions resulting in high mobility of condensing water droplets. A large increase of the ensuing ice coverage time is shown compared to the cases of standard smooth hydrophilic or textured superhydrophobic surfaces. During deicing of these self-impregnating surfaces we show an impressive tendency of ice fragments to skate expediting defrosting. Robustness of such surfaces is also demonstrated by operating them under subcooling for at least 490hr without a marked degradation. This is attributed to the presence of the liquid intervening layer, which protects the substrate from hydrolyzation enhancing longevity and sustaining heat transfer efficiency.",1703.07349v1 2019-02-03,Non-monotonic pressure dependence of high-field nematicity and magnetism in CeRhIn$_5$,"CeRhIn$_5$ provides a textbook example of quantum criticality in a heavy fermion system: Pressure suppresses local-moment antiferromagnetic (AFM) order and induces superconductivity in a dome around the associated quantum critical point (QCP) near $p_{c} \approx 23\,$kbar. Strong magnetic fields also suppress the AFM order at a field-induced QCP at $B_{\rm c}\approx 50\,$T. In its vicinity, a nematic phase at $B^*\approx 28\,$T characterized by a large in-plane resistivity anisotropy emerges. Here, we directly investigate the interrelation between these phenomena via magnetoresistivity measurements under high pressure. As pressure increases, the nematic transition shifts to higher fields, until it vanishes just below $p_{\rm c}$. While pressure suppresses magnetic order in zero field as $p_{\rm c}$ is approached, we find magnetism to strengthen under strong magnetic fields due to suppression of the Kondo effect. We reveal a strongly non-mean-field-like phase diagram, much richer than the common local-moment description of CeRhIn$_5$ would suggest.",1902.00970v3 2020-02-11,Observation of an antiferromagnetic quantum critical point in high-purity LaNiO$_3$,"Amongst the rare-earth perovskite nickelates, LaNiO$_3$ (LNO) is an exception. While the former have insulating and antiferromagnetic ground states, LNO remains metallic and non-magnetic down to the lowest temperatures. It is believed that LNO is a strange metal, on the verge of an antiferromagnetic instability. Our work suggests that LNO is a quantum critical metal, close to an antiferromagnetic quantum critical point (QCP). The QCP behavior in LNO is manifested in epitaxial thin films with unprecedented high purities. We find that the temperature and magnetic field dependences of the resistivity of LNO at low temperatures are consistent with scatterings of charge carriers from weak disorder and quantum fluctuations of an antiferromagnetic nature. Furthermore, we find that the introduction of a small concentration of magnetic impurities qualitatively changes the magnetotransport properties of LNO, resembling that found in some heavy-fermion Kondo lattice systems in the vicinity of an antiferromagnetic QCP.",2002.04159v1 2020-09-18,Nanoscale structural and electrical properties of graphene grown on AlGaN by catalyst-free chemical vapor deposition,"The integration of graphene (Gr) with nitride semiconductors is highly interesting for applications in high-power/high-frequency electronics and optoelectronics. In this work, we demonstrated the direct growth of Gr on Al0.5Ga0.5N/sapphire templates by propane (C3H8) chemical vapor deposition (CVD) at temperature of 1350{\deg}C. After optimization of the C3H8 flow rate, a uniform and conformal Gr coverage was achieved, which proved beneficial to prevent degradation of AlGaN morphology. X-ray photoemission spectroscopy (XPS) revealed Ga loss and partial oxidation of Al in the near-surface AlGaN region. Such chemical modification of a 2 nm thick AlGaN surface region was confirmed by cross-sectional scanning transmission electron microscopy (STEM) combined with electron energy loss spectroscopy (EELS), which also showed the presence of a bilayer of Gr with partial sp2/sp3 hybridization. Raman spectra indicated that the deposited Gr is nanocrystalline (with domain size 7 nm) and compressively strained. A Gr sheet resistance of 15.8 kOhm/sq was evaluated by four-point-probe measurements, consistently with the nanocrystalline nature of these films. Furthermore, nanoscale resolution current mapping by conductive atomic force microscopy (C-AFM) indicated local variations of the Gr carrier density at a mesoscopic scale, which can be ascribed to changes in the charge transfer from the substrate due to local oxidation of AlGaN or to the presence of Gr wrinkles.",2009.08673v1 2017-07-28,3D laser printing by ultra-short laser pulses for micro-optical applications: towards telecom wavelengths,"Three dimensional (3D) fast (< 0.5 hour) printing of micro-optical elements down to sub-wavelength resolution over 100 micrometers footprint areas using femtosecond (fs-)laser oscillator is presented. Using sub-1 nJ pulse energies, optical vortex generators made of polymerised grating segments with an azimuthally changing orientation have been fabricated in SZ2080 resist; width of polymerised rods was ~150 nm and period 0.6-1 micrometers. Detailed phase retardance analysis was carried out manually with Berek compensator (under a white light illumination) and using an equivalent principle by an automated Abrio implementation at 546 nm. Direct experimental measurements of retardance was required since the period of the grating was comparable (or larger) than the wavelength of visible light. By gold sputtering, transmission-type optical vortex generators were turned into reflective ones with augmented retardance, n.h defined by the form birefringence, n, and the height h = 2d where d is the thickness of the polymerised structure. Retardance reached 315 nm as measured with Berek compensator at visible wavelengths. Birefringent phase delays of 180 degrees (or half-wavelength) required for high purity vortex generators can be made based on the proposed approach. Optical vortex generators for telecom wavelengths with sub-wavelength patterns of azimuthally oriented gratings are amenable by direct laser polymerisation.",1707.09365v1 2017-08-14,High-Kinetic Inductance Additive Manufactured Superconducting Microwave Cavity,"Investigations into the microwave surface impedance of superconducting resonators have led to the development of single photon counters that rely on kinetic inductance for their operation. While concurrent progress in additive manufacturing, `3D printing', opens up a previously inaccessible design space for waveguide resonators. In this manuscript, we present results from the first synthesis of these two technologies in a titanium, aluminum, vanadium (Ti-6Al-4V) superconducting radio frequency resonator which exploits a design unattainable through conventional fabrication means. We find that Ti-6Al-4V has two distinct superconducting transition temperatures observable in heat capacity measurements. The higher transition temperature is in agreement with DC resistance measurements. While the lower transition temperature, not previously known in literature, is consistent with the observed temperature dependence of the superconducting microwave surface impedance. From the surface reactance, we extract a London penetration depth of $8\pm3{\mu}$m - roughly an order of magnitude larger than other titanium alloys and several orders of magnitude larger than other conventional elemental superconductors. This large London penetration depth suggests that Ti-6Al-4V may be a suitable material for high kinetic inductance applications such as single photon counting or parametric amplification used in quantum computing.",1708.04273v1 2018-08-13,Ultra-compact graphene plasmonic photodetector with the bandwidth over 110GHz,"Graphene-based photodetectors, taking advantage of high carrier mobility and broadband absorption in graphene, have recently experienced rapid development. However, their performances with respect to the responsivity and bandwidth are still limited by either weak light-graphene interaction or large resistance-capacitance product. Here, we demonstrate a waveguide coupled integrated graphene plasmonic photodetector on the silicon-on-insulator platform. Benefiting from plasmonic enhanced graphene-light interactions and subwavelength confinement of the optical energy, we present a small-footprint graphene-plasmonic photodetector with bandwidth beyond 110GHz and intrinsic responsivity of 360mA/W. Attributed to the unique electronic bandstructure of graphene and its ultra-broadband absorption, the operational wavelength range extending beyond mid-infrared, and possibly further, can be anticipated. Our results show that the combination of graphene with plasmonic devices has great potential to realize ultra-compact and high-speed optoelectronic devices for graphene-based optical interconnects.",1808.04815v3 2019-03-22,Structure and mechanical behavior of ultrafine-grained aluminum-iron alloy stabilized by nanoscaled intermetallic particles,"Ultrafine-grained aluminum alloys offer interesting multifunctional properties with a combination of high strength, low electrical resistivity, and low density. However, due to thermally induced grain coarsening, they typically suffer from an intrinsic poor thermal stability. To overcome this drawback, an Al-2%Fe alloy has been selected because of the low solubility of Fe in Al and their highly positive enthalpy of mixing leading to the formation of stable intermetallic particles. The two-phase alloy has been processed by severe plastic deformation to achieve simultaneously submicrometer Al grains and a uniform distribution of nanoscaled intermetallic particles. The influence of the level of deformation on the microstructure has been investigated thanks to transmission electron microscopy and atom probe tomography and it is shown that for the highest strain a partial dissolution of the metastable Al6Fe particle occurred leading to the formation of a Fe super saturated solid solution. The thermal stability, and especially the precipitation of particles from the ultrafine-grained solid solution and the way they pin grain boundaries has been investigated both from static annealing and in-situ transmission electron microscopy experiments. The correlation between microstructural features and microhardness has been established to identify the various strengthening contributions. Finally, it is 2 shown that ultrafine grained high purity Al with less than 0.01 at. % Fe in solid solution could preserve a grain size only 300nm after 1h at 250$^\circ$C.",1903.09391v1 2019-03-27,Homogeneous hierarchical NiMoO4@NiMoO4 nanostructure as a high-performance anode material for electrochemical energy storage,"Here we report the extraordinary electrochemical energy storage capability of NiMoO4@NiMoO4 homogeneous hierarchical nanosheet-on-nanowire-arrays (SOWAs) synthesized on nickel substrate by a two-stage hydrothermal process. Comparatively speaking, the SOWAs electrode displays improved electrochemical performances than the bare NiMoO4 nanowire arrays. Such improvements can be ascribed to the characteristic homogeneous hierarchical structure which not only effectively increases the active surface areas for fast charge transfer, but also reduces the electrode resistance significantly by eliminating the potential barrier at the nanowire/nanosheet junction, which is usually an issue in other reported heterogeneous architectures. We further evaluate the performances of the SOWAs by constructing an asymmetric hybrid supercapacitor (ASC) with the SOWAs and activated carbon (AC). The optimized ASC shows excellent electrochemical performances with 47.2 Wh/kg in energy density at 1.38 kW/kg at 0-1.2 V. Moreover, the specific capacity retention can be as high as 91.4% after 4000 cycles, illustrating the remarkable cycling stability of the NiMoO4@NiMoO4//AC ASC device. Our results show that this unique NiMoO4@NiMoO4 SOWAs display great prospect for future energy storage applications",1903.11513v1 2019-04-29,Type-II Ising superconductivity and anomalous metallic state in macro-size ambient-stable ultrathin crystalline films,"Recent emergence of two-dimensional (2D) crystalline superconductors has provided a promising platform to investigate novel quantum physics and potential applications. To reveal essential quantum phenomena therein, ultralow temperature transport investigation on high quality ultrathin superconducting films is critically required, although it has been quite challenging experimentally. Here we report a systematic transport study on the ultrathin crystalline PdTe2 films grown by molecular beam epitaxy (MBE). Interestingly, a new type of Ising superconductivity in 2D centrosymmetric materials is revealed by the detection of large in-plane critical field more than 7 times Pauli limit. Remarkably, in perpendicular magnetic field, we provide solid evidence of anomalous metallic state characterized by the resistance saturation at low temperatures with high quality filters. The robust superconductivity with intriguing quantum phenomena in the macro-size ambient-stable ultrathin PdTe2 films remains almost the same for 20 months, showing great potentials in electronic and spintronic applications.",1904.12719v2 2016-09-08,Evidence of Ballistic Thermal Transport in Lithium Niobate at Room Temperature,"In ballistic transport, heat carriers such as phonons travel through the solid without any scattering or interaction. Therefore, there is no temperature gradient in the solid, which seems to transport the heat without getting heated itself. Ballistic transport is typically seen in high purity crystals at either temperatures below ~10 K, or physical size below ~100 nm, where the mean free path of the carrier is larger than the solid itself. In this letter, we show evidence of ballistic transport at room temperature in lithium niobate wafers in the in-plane and cross-plane directions under both steady state and high frequency heating that are monitored using both infrared and resistance thermometry. We report phonon mean free path in lithium niobate around 425 microns, which is about 50 times higher than the largest phonon mean free path in the literature at room temperature. Above this length-scale, temperature gradient gradually emerges and the material shows completely diffusive, bulk transport at about 4 mm length. Our observations will impact phonon-based electronics such as thermal transistor, thermal logic gate and memory currently impossible at room temperature. If 1 micron electron mean free path in graphene gives the highest-mobility, the 425 microns mean free path of phonons in this research may realize phononics without any need for nanoscale size or ultra-cold temperatures.",1609.02585v1 2018-07-03,ssDNA sequencing by rectification,"Fast, reliable and inexpensive DNA sequencing is an important pursuit in healthcare, especially in personalized medicine with possible deep societal impacts. Despite significant progress of various nanopore-based sequencing configurations, challenges remain in resolution (due to thermal fluctuations or to sensitivity to molecular orientation) and speed, which are calling for new approaches. Here we propose a sequencing protocol for DNA translocation through a nanopore with side-embedded N-terminated carbon nanotube electrodes. Employing DFT and Non-Equilibrium Green's Function formalism, we show that the rectification ratio (response to square pulses of alternating bias) bears high nucleobase specificity. The rectification arises due to bias-dependent resistance asymmetry on the deoxyribonucleotide-electrode interfaces. The asymmetry induces molecular charging and HOMO pinning to the electrochemical potential of one of the electrodes, assisted by an in-gap electric field effect caused by dipoles at the terminated electrode ends. This sequencing protocol is sensitive, selective with orders of magnitude, has high resolution, and it is robust to molecular orientation.",1807.01215v4 2018-12-16,Quantum dots formed in three-dimensional Dirac semimetal Cd$_3$As$_2$ nanowires,"We demonstrate quantum dot (QD) formation in three-dimensional Dirac semimetal Cd$_{3}$As$_{2}$ nanowires using two electrostatically tuned p$-$n junctions with a gate and magnetic fields. The linear conductance measured as a function of gate voltage under high magnetic fields is strongly suppressed at the Dirac point close to zero conductance, showing strong conductance oscillations. Remarkably, in this regime, the Cd$_{3}$As$_{2}$ nanowire device exhibits Coulomb diamond features, indicating that a clean single QD forms in the Dirac semimetal nanowire. Our results show that a p$-$type QD can be formed between two n$-$type leads underneath metal contacts in the nanowire by applying gate voltages under strong magnetic fields. Analysis of the quantum confinement in the gapless band structure confirms that p$-$n junctions formed between the p$-$type QD and two neighboring n$-$type leads under high magnetic fields behave as resistive tunnel barriers due to cyclotron motion, resulting in the suppression of Klein tunneling. The p$-$type QD with magnetic field-induced confinement shows a single hole filling. Our results will open up a route to quantum devices such as QDs or quantum point contacts based on Dirac and Weyl semimetals.",1812.06416v1 2019-01-17,Compositional dependence of epitaxial Tin+1SiCn MAX-phase thin films grown from a Ti3SiC2 compound target,"We investigate sputtering of a Ti3SiC2 compound target at temperatures ranging from RT (no applied external heating) to 970 oC as well as the influence of the sputtering power at 850 oC for the deposition of Ti3SiC2 films on Al2O3(0001) substrates. Elemental composition obtained from time-of-flight energy elastic recoil detection analysis shows an excess of carbon in all films, which is explained by differences in angular distribution between C, Si and Ti, where C scatters the least during sputtering. The oxygen content is 2.6 at.% in the film deposited at RT and decreases with increasing deposition temperature, showing that higher temperatures favor high purity films. Chemical bonding analysis by X-ray photoelectron spectroscopy shows C-Ti and Si-C bonding in the Ti3SiC2 films and Si-Si bonding in the Ti3SiC2 compound target. X-ray diffraction reveals that the phases Ti3SiC2, Ti4SiC3, and Ti7Si2C5 can be deposited from a Ti3SiC2 compound target at substrate temperatures above 850 oC and with growth of TiC and the Nowotny phase Ti5Si3Cx at lower temperatures. High-resolution scanning transmission electron microscopy shows epitaxial growth of Ti3SiC2, Ti4SiC3, and Ti7Si2C5 on TiC at 970 oC. Four-point probe resistivity measurements give values in the range 120 to 450 micro-Ohm-cm and with the lowest values obtained for films containing Ti3SiC2, Ti4SiC3, and Ti7Si2C5.",1901.05904v1 2019-06-10,Anomalous electron transport in epitaxial NdNiO$_3$ films,"The origin of simultaneous electronic, structural and magnetic transitions in bulk rare-earth nickelates ($RE$NiO$_3$) remains puzzling with multiple conflicting reports on the nature of these entangled phase transitions. Heterostructure engineering of these materials offers unique opportunity to decouple metal-insulator transition (MIT) from the magnetic transition. However, the evolution of underlying electronic properties across these decoupled transitions remains largely unexplored. In order to address this, we have measured Hall effect on a series of epitaxial NdNiO$_3$ films, spanning a variety of electronic and magnetic phases. We find that the MIT results in only partially gapped Fermi surface, whereas full insulating phase forms below the magnetic transition. In addition, we also find a systematic reduction of the Hall coefficient ($R_H$) in the metallic phase of these films with epitaxial strain and also a surprising transition to negative value at large compressive strain. Partially gapped weakly insulating, paramagnetic phase is reminiscence of pseudogap behavior of high $T_c$ cuprates. The precursor metallic phase, which undergoes transition to insulating phase is a non-Fermi liquid with the temperature exponent ($n$) of resistivity of 1, whereas the exponent increases to 4/3 in the non-insulating samples. Such nickelate phase diagram with sign-reversal of $R_H$, pseudo-gap phase and non Fermi liquid behavior are intriguingly similar to high $T_c$ cuprates, giving important guideline to engineer unconventional superconductivity in oxide heterostructure.",1906.03809v1 2019-10-22,Magnetic topological insulator MnBi6Te10 with zero-field ferromagnetic state and gapped Dirac surface states,"Magnetic topological insulators (TIs) with nontrivial topological electronic structure and broken time-reversal symmetry exhibit various exotic topological quantum phenomena. The realization of such exotic phenomena at high temperature is one of central topics in this area. We reveal that MnBi6Te10 is a magnetic TI with an antiferromagnetic ground state below 10.8 K whose nontrivial topology is manifested by Dirac-like surface states. The ferromagnetic axion insulator state with Z4 = 2 emerges once spins polarized at field as low as 0.1 T, accompanied with saturated anomalous Hall resistivity up to 10 K. Such a ferromagnetic state is preserved even external field down to zero at 2 K. Theoretical calculations indicate that the few-layer ferromagnetic MnBi6Te10 is also topologically nontrivial with a non-zero Chern number. Angle-resolved photoemission spectroscopy experiments further reveal three types of Dirac surface states arising from different terminations on the cleavage surfaces, one of which has insulating behavior with an energy gap of ~ 28 meV at the Dirac point. These outstanding features suggest that MnBi6Te10 is a promising system to realize various topological quantum effects at zero field and high temperature.",1910.10101v2 2020-01-03,Coulomb Blockade Effects in a Topological Insulator Grown on a High-Tc Cuprate Superconductor,"The evidence for proximity-induced superconductivity in heterostructures of topological insulators and high-Tc cuprates has been intensely debated. We use molecular beam epitaxy to grow thin films of topological insulator Bi2Te3 on a cuprate Bi2Sr2CaCu2O8+x, and study the surface of Bi2Te3 using low-temperature scanning tunneling microscopy and spectroscopy. In few unit-cell thick Bi2Te3 films, we find a V-shaped gap-like feature at the Fermi energy in dI/dV spectra. By reducing the coverage of Bi2Te3 films to create nanoscale islands, we discover that this spectral feature dramatically evolves into a much larger hard gap, which can be understood as a Coulomb blockade gap. This conclusion is supported by the evolution of dI/dV spectra with the lateral size of Bi2Te3 islands, as well as by topographic measurements that show an additional barrier separating Bi2Te3 and Bi2Sr2CaCu2O8+x. We conclude that the prominent gap-like feature in dI/dV spectra in Bi2Te3 films is not a proximity-induced superconducting gap. Instead, it can be explained by Coulomb blockade effects, which take into account additional resistive and capacitive coupling at the interface. Our experiments provide a fresh insight into the tunneling measurements of complex heterostructures with buried interfaces.",2001.00906v2 2020-07-14,Cyclic plasticity and fatigue damage of CrMnFeCoNi high entropy alloy fabricated by laser powder-bed fusion,"The CrMnFeCoNi high-entropy alloy is highly printable and holds great potential for structural applications. However, no significant discussions on cyclic plasticity and fatigue damage in previous studies. This study provides significant insights into the link between print processes, solidification microstructure, cyclic plasticity and fatigue damage evolution in the alloy fabricated by laser powder bed fusion. Thermodynamics-based predictions (validated by scanning transmission electron microscopy (STEM) energy dispersive X-ray spectroscopy (EDX)) showed that Cr, Co and Fe partition to the core of the solidification cells, whilst Mn and Ni to the cell boundaries in all considered print parameters. Both dislocation slip and deformation twinning were found to be responsible for plastic deformation under monotonic loading. However, the former was found to be the single dominant mechanism for cyclic plasticity. The surface finish helped to substantially delay the crack initiation and cause lack-of-fusion porosity to be the main source of crack initiation. Most significantly, the scan strategies significantly affect grain arrangements and grain dimensions, leading to noticeable effects on fatigue crack propagation; in particular, the highest resistance crack propagation was seen in the meander scan strategy with 0{\deg} rotation thanks to the most columnar grains and the smallest spacing of grain boundaries along the crack propagation path.",2007.07043v1 2020-07-24,Integration of multi-layer black phosphorus into photoconductive antennas for THz emission,"We report the fabrication, characterization, and modeling of photoconductive antennas using 40 nm thin-film flakes of black phosphorus (BP) as the photoconductor and hexagonal boron nitride (hBN) as a capping layer to prevent oxidation of BP. Dipole antennas were fabricated on oxidized high-resistivity Si substrates, and BP and hBN flakes were picked up and transferred onto the antenna inside a nitrogen glovebox. The transfer matrix technique was used to optimize the thickness of BP and hBN for maximum absorption. BP flakes were aligned with the armchair axis along the anode-cathode gap of the antenna, with crystal orientation measured using reflection anisotropy. Photocurrent imaging under illumination with 100 fs pulses at 780 and 1560 nm showed a bias-dependent maximum photocurrent localized to the antenna gap with a peak photoconductivity of 1 (2) S/cm in the linear regime of bias for excitation at 780 (1560) nm. Photocurrent saturation in bias (pump fluence) occurred at approximately 1 V (0.25 mJ/cm$^2$). Device performance was modeled numerically by solving Maxwell's equations and the drift-diffusion equation to obtain the photocurrent density in response to pulsed laser excitation, which was largely in qualitative agreement with the experimental observations. THz output computed from surface current density suggests that BP THz PCA performance is at least comparable to more traditional devices based on low-temperature-grown GaAs. These devices represent a step toward high-performance THz photoconductive antennas using BP.",2007.12775v1 2020-08-06,Constraining the ellipticity of millisecond pulsars with observed spin-down rates,"A spinning neutron star (NS) that is asymmetric with respect to its spin axis can emit continuous gravitational wave (GW) signals. The spin frequencies and their distribution of radio millisecond pulsars (MSPs) and accreting MSPs provide some evidences of GW radiation, and MSPs are ideal probes detecting high frequency GW signals. It is generally thought that MSPs originate from the recycled process, in which the NS accretes the material and angular momentum from the donor star. The accreted matter would be confined at the polar cap zone by an equatorial belt of compressed magnetic field fixed in the deep crust of the NS, and yields ""magnetic mountain"". Based on an assumption that the spin-down rates of three transitional MSPs including PSR J1023+0038 are the combinational contribution of the accretion torque, the propeller torque, and the GW radiation torque, in this work we attempt to constrain the ellipticities of MSPs with observed spin-down rates. Assuming some canonical parameters of NSs, the ellipticities of three transitional MSPs and ten redbacks are estimated to be $\epsilon=(0.9-23.4)\times 10^{-9}$. The electrical resistivities of three transitional MSPs are also derived to be in the range $\eta=(1.2-15.3)\times 10^{-31}~\rm s$, which display an ideal power law relation with the accretion rate. The characteristic strains ($h_{\rm c}=(0.6-2.5)\times10^{-27}$) of GW signals emitting by these sources are obviously beyond the sensitivity scope of the aLIGO. We expect that the third-generation GW detectors like the Einstein Telescope can seize the GW signals from these sources in the future.",2008.02444v2 2020-08-22,Large Transport Gap Modulation in Graphene via Electric Field Controlled Reversible Hydrogenation,"Graphene is of interest in the development of next-generation electronics due to its high electron mobility, flexibility and stability. However, graphene transistors have poor on/off current ratios because of the absence of a bandgap. One approach to introduce an energy gap is to use hydrogenation reaction, which changes graphene into insulating graphane with sp3 bonding. Here we show that an electric field can be used to control conductor-to-insulator transitions in microscale graphene via a reversible electrochemical hydrogenation in an organic liquid electrolyte containing dissociative hydrogen ions. The fully hydrogenated graphene exhibits a lower limit sheet resistance of 200 Gohm/sq, resulting in graphene field-effect transistors with on/off current ratios of 10^8 at room temperature. The devices also exhibit high endurance, with up to one million switching cycles. Similar insulating behaviours are also observed in bilayer graphene, while trilayer graphene remains highly conductive after the hydrogenation. Changes in the graphene lattice, and the transformation from sp2 to sp3 hybridization, is confirmed by in-situ Raman spectroscopy, supported by first-principles calculations.",2008.09749v2 2020-10-04,Ballistic-hydrodynamic phase transition in flow of two-dimensional electrons,"Phase transitions are characterized by a sharp change in the type of dynamics of microparticles, and their description usually requires quantum mechanics. Recently, a peculiar type of conductors was discovered in which two-dimensional (2D) electrons form a viscous fluid. In this work we reveal that such electron fluid in high-quality samples can be formed from ballistic electrons via a phase transition. For this purpose, we theoretically study the evolution of a ballistic flow of 2D weakly interacting electrons with an increase of magnetic field and trace an emergence of a fluid fraction at a certain critical field. Such restructuring of the flow manifests itself in a kink in magnetic-field dependencies of the longitudinal and the Hall resistances. It is remarkable that the studied phase transition has a classical-mechanical origin and is determined by both the ballistic size effects and the electron-electron scattering. Our analysis shows that this effect was apparently observed in the recent transport experiments on 2D electrons in graphene and high-mobility GaAs quantum wells.",2010.01642v4 2020-10-22,Li-ion Battery Fault Detection in Large Packs Using Force and Gas Sensors,"Internal short circuits are a leading cause of battery thermal runaway, and hence a major safety issue for electric vehicles. An internal short circuit with low resistance is called a hard internal short, which causes a high internal current flow that leads to an extremely fast temperature rise, gas generation, cell swelling, and ultimately battery rupture and failure. Thus it is crucial to detect these faults immediately after they get triggered. In large battery packs with many cells in parallel, detecting an internal short circuit event using voltage is difficult due to suppression of the voltage signal from the faulty cell by the other healthy cells connected in parallel. In contrast, analyzing the gas composition in the pack enclosure can provide a robust single cell failure detection method. At elevated temperature, decomposition of the battery materials results in gas generation and cell swelling. The cell structure is designed to rupture at a critical gas pressure and vent the accumulated $CO_2$ gas, in order to prevent explosive forces. In this paper, we extend our previous work by combining the models of cell thermal dynamics, swelling, and $CO_2$ gas generation. In particular, we developed a fast and high confidence level detection method of hard internal short circuit events for a battery pack by measuring cell expansion force and monitoring $CO_2$ concentrations in a pack enclosure.",2010.13519v1 2020-11-01,Experimental demonstration of particle acceleration with normal conducting accelerating structure at cryogenic temperature,"Reducing the operating temperature of normal conducting particle accelerators substantially increases their efficiency. Low-temperature operation increases the yield strength of the accelerator material and reduces surface resistance, hence a great reduction in cyclic fatigue could be achieved resulting in a large reduction in breakdown rates compared to room-temperature operation. Furthermore, temperature reduction increases the intrinsic quality factor of the accelerating cavities, and consequently, the shunt impedance leading to increased system efficiency and beam loading capabilities. In this paper, we present an experimental demonstration of the high-gradient operation of an X-band, 11.424 GHz, 20-cells linear accelerator (linac) operating at a liquid nitrogen temperature of 77 K. The tested linac was previously processed and tested at room temperature. We verified the enhanced accelerating parameters of the tested accelerator at cryogenic temperature using different measurements including electron beam acceleration up to a gradient of 150 MV/m, corresponding to a peak surface electric field of 375 MV/m. We also measured the breakdown rates in the tested structure showing a reduction of two orders of magnitude, x100, compared to their values at room temperature for the same accelerating gradient.",2011.00391v1 2020-12-13,Microfluidic device coupled with total internal reflection microscopy for in situ observation of precipitation,"In situ observation of precipitation or phase separation induced by solvent addition is important in studying its dynamics. Combined with optical and fluorescence microscopy, microfluidic devices have been leveraged in studying the phase separation in various materials including biominerals, nanoparticles, and inorganic crystals. However, strong scattering from the subphases in the mixture is problematic for in situ study of phase separation with high temporal and spatial resolution. In this work, we present a quasi-2D microfluidic device combined with total internal reflection microscopy as an approach for in situ observation of phase separation. The quasi-2D microfluidic device comprises of a shallow main channel and a deep side channel. Mixing between a solution in the main channel (solution A) and another solution (solution B) in the side channel is predominantly driven by diffusion due to high fluid resistance from the shallow height of the main channel, which is confirmed using fluorescence microscopy. Moreover, relying on diffusive mixing, we can control the composition of the mixture in the main channel by tuning the composition of solution B. We demonstrate the application of our method for in situ observation of asphaltene precipitation and beta-alanine crystallization.",2012.06962v1 2021-01-31,Monoclinic EuSn$_2$As$_2$: A Novel High-Pressure Network Structure,"The layered crystal of EuSn$_2$As$_2$ has a Bi$_2$Te$_3$-type structure in rhombohedral ($R\bar{3}m$) symmetry and has been confirmed to be an intrinsic magnetic topological insulator at ambient conditions. Combining {\it ab initio} calculations and \emph{in-situ} x-ray diffraction measurements, we identify a new monoclinic EuSn$_2$As$_2$ structure in $C2/m$ symmetry above $\sim$14 GPa. It has a three-dimensional network made up of honeycomb-like Sn sheets and zigzag As chains, transformed from the layered EuSn$_2$As$_2$ via a two-stage reconstruction mechanism with the connecting of Sn-Sn and As-As atoms successively between the buckled SnAs layers. Its dynamic structural stability has been verified by phonon mode analysis. Electrical resistance measurements reveal an insulator-metal-superconductor transition at low temperature around 5 and 15 GPa, respectively, according to the structural conversion, and the superconductivity with a \textit{T}${\rm {_C}}$ value of $\sim 4$ K is observed up to 30.8 GPa. These results establish a high-pressure EuSn$_2$As$_2$ phase with intriguing structural and electronic properties and expand our understandings about the layered magnetic topological insulators.",2102.00437v2 2021-02-18,Crystal orientation-dependent oxidation of epitaxial TiN films with tunable plasmonics,"Titanium nitride (TiN) is a paradigm of refractory transition metal nitrides with great potential in vast applications. Generally, the plasmonic performance of TiN can be tuned by oxidation, which was thought to be only temperature-, oxygen partial pressure-, and time-dependent. Regarding the role of crystallographic orientation in the oxidation and resultant optical properties of TiN films, little is known thus far. Here we reveal that both the oxidation resistance behavior and the plasmonic performance of epitaxial TiN films follow the order of (001) < (110) < (111). The effects of crystallographic orientation on the lattice constants, optical properties, and oxidation levels of epitaxial TiN films have been systematically studied by combined high-resolution X-ray diffraction, spectroscopic ellipsometry, X-ray absorption spectroscopy, and X-ray photoemission spectroscopy. To further understand the role of crystallographic orientation in the initial oxidation process of TiN films, density-functional-theory calculations are carried out, indicating the energy cost of oxidation is (001) < (110) < (111), consistent with the experiments. The superior endurance of the (111) orientation against mild oxidation can largely alleviate the previously stringent technical requirements for the growth of TiN films with high plasmonic performance. The crystallographic orientation can also offer an effective controlling parameter to design TiN-based plasmonic devices with desired peculiarity, e.g., superior chemical stability against mild oxidation or large optical tunability upon oxidation.",2102.09126v1 2021-03-15,Thermal Visualization of Buried Interfaces by Transient and Steady-State Responses of Time-Domain Thermoreflectance,"Thermal resistances from interfaces impede heat dissipation in micro/nanoscale electronics, especially for high-power electronics. Despite the growing importance of understanding interfacial thermal transport, advanced thermal characterization techniques which can visualize thermal conductance across buried interfaces, especially for nonmetal-nonmetal interfaces, are still under development. This work reports a dual-modulation-frequency TDTR mapping technique to visualize the thermal conduction across buried semiconductor interfaces for beta-Ga2O3-SiC samples. Both the beta-Ga2O3 thermal conductivity and the buried beta-Ga2O3-SiC thermal boundary conductance (TBC) are visualized for an area of 200 um x 200 um. Areas with low TBC values ( smaller than 20 MW/m2-K) are successfully identified on the TBC map, which correspond to weakly bonded interfaces caused by high-temperature annealing. The steady-state temperature rise (detector voltage), usually ignored in TDTR measurements, is found to be able to probe TBC variations of the buried interfaces without the limit of thermal penetration depth. This technique can be applied to detect defects/voids in deeply buried heterogeneous interfaces non-destructively, and also opens a door for the visualization of thermal conductance in nanoscale nonhomogeneous structures.",2103.08084v1 2021-03-24,Quantum transport properties of beta-Bi4I4 near and well beyond the extreme quantum limit,"We have investigated the magneto-transport properties of beta-Bi4I4 bulk crystal, which was recently theoretically proposed and experimentally demonstrated to be a topological insulator. At low temperature T and magnetic field B, a series of Shubnikov-De Haas(SdH) oscillations are observed on the magnetoresistivity (MR). The detailed analysis reveals a light cyclotron mass of 0.1 me, and the field angle dependence of MR reveals that the SdH oscillations originate from a convex Fermi surface. In the extreme quantum limit (EQL) region, there is a metal-insulator transition occurring soon after the EQL. We perform the scaling analysis, and all the isotherms fall onto a universal scaling with a fitted critical exponent of 6.5. The enormous value of critical exponent implies this insulating quantum phase originated from strong electron-electron interactions in high fields. However, in the far end of EQL, both the longitudinal and Hall resistivity increase exponentially with B, and the temperature dependence of the MR reveals an energy gap induced by the high magnetic field, signifying a magnetic freeze-out effect. Our findings indicate that bulk beta-Bi4I4 is an excellent candidate for a 3D topological system for exploring EQL physics and relevant exotic quantum phases.",2103.13079v2 2021-04-15,"Negligible oxygen vacancies, low critical current density, electric-field modulation, in-plane anisotropic and high-field transport of a superconducting Nd0.8Sr0.2NiO2/SrTiO3 heterostructure","The emerging Ni-based superconducting oxide thin films are rather intriguing to the entire condensed matter physics. Here we report some brief experimental results on transport measurements for a 14-nm-thick superconducting Nd0.8Sr0.2NiO2/SrTiO3 thin-film heterostructure with an onset transition temperature of ~9.5 K. Photoluminescence measurements reveal that there is negligible oxygen vacancy creation in the SrTiO3 substrate during thin-film deposition and post chemical reduction for the Nd0.8Sr0.2NiO2/SrTiO3 heterostructure. It was found that the critical current density of the Nd0.8Sr0.2NiO2/SrTiO3 thin-film heterostructure is relatively small, ~4x10^3 A/cm2. Although the surface steps of SrTiO3 substrates lead to an anisotropy for in-plane resistivity, the superconducting transition temperatures are almost the same. The out-of-plane magnetotransport measurements yield an upper critical field of ~11.4 T and an estimated in-plane Ginzburg-Landau coherence length of ~5.4 nm. High-field magnetotransport measurements up to 50 T reveal anisotropic critical fields at 1.8 K for three different measurement geometries and a complicated Hall effect. An electric field applied via the SrTiO3 substrate slightly varies the superconducting transition temperature. These experimental results could be useful for this rapidly developing field.",2104.07316v2 2021-04-26,Impact of the nucleation of charge clusters on the retention of memristors: a self-consistent phase field computational study,"In recent years, resistive RAM often referred to as memristor is actively pursued as a replacement for nonvolatile-flash memory due to its superior characteristics such as high density, scalability, low power operation, high endurance, and fast operating speed. However, one of the challenges that need to be overcome is the loss of retention for both ON- and OFF-states; the retention loss. While various models are proposed to explain the retention loss in memristors consisting of a switching layer, in this paper, we propose that the nucleation of clusters made of electrical charges, charge-clusters, in the switching layer acts as a potential root cause for the retention loss. The nucleation results from localized electric-field produced intermittently during cyclic switching operations. We use the phase-field method to illustrate how the nucleation of charge-clusters gives rise to the retention loss. Our results suggest that the degree at which the retention loss arises is linked to the number of cyclic switching operations since the probability at which nucleation centers form increases with the number of cycle switching operations, which is consistent with a range of experimental findings previously reported.",2104.12829v1 2021-06-02,Multiband effects on the upper critical field angular dependence of 122-family iron pnictide superconductors,"Detailed measurements of the in-plane resistivity were performed in a high-quality Ba(Fe$_{1-x}$Co$_{x}$)$_2$As$_2$ ($x=0.065$) single crystal, in magnetic fields up to 9 T and with different orientations $\theta$ relative to the crystal $c$ axis. A significant $\rho(T)_{H,\theta}$ rounding is observed just above the superconducting critical temperature $T_c$ due to Cooper pairs created by superconducting fluctuations. These data are analyzed in terms of a generalization of the Aslamazov-Larkin approach, that extends its applicability to high reduced-temperatures and magnetic fields. This method allows us to carry out a criterion-independent determination of the angular dependence of the upper critical field, $H_{c2}(\theta)$. In spite of the relatively small anisotropy of this compound, it is found that $H_{c2}(\theta)$ presents a significant deviation from the single-band 3D anisotropic Ginzburg-Landau (3D-aGL) approach, particularly for large $\theta$ (typically above $\sim60^o$). These results are interpreted in terms of the multiband nature of these materials, in contrast with other proposals for similar $H_{c2}(\theta)$ anomalies. Our results are also consistent with an effective anisotropy factor almost temperature independent near $T_c$, a result that differs from the ones obtained by using a single-band model.",2106.01307v1 2021-07-07,Magnetization-tuned topological quantum phase transition in MnBi2Te4 devices,"Recently, the intrinsic magnetic topological insulator MnBi2Te4 has attracted enormous research interest due to the great success in realizing exotic topological quantum states, such as the quantum anomalous Hall effect (QAHE), axion insulator state, high-Chern-number and high-temperature Chern insulator states. One key issue in this field is to effectively manipulate these states and control topological phase transitions. Here, by systematic angle-dependent transport measurements, we reveal a magnetization-tuned topological quantum phase transition from Chern insulator to magnetic insulator with gapped Dirac surface states in MnBi2Te4 devices. Specifically, as the magnetic field is tilted away from the out-of-plane direction by around 40-60 degrees, the Hall resistance deviates from the quantization value and a colossal, anisotropic magnetoresistance is detected. The theoretical analyses based on modified Landauer-Buttiker formalism show that the field-tilt-driven switching from ferromagnetic state to canted antiferromagnetic state induces a topological quantum phase transition from Chern insulator to magnetic insulator with gapped Dirac surface states in MnBi2Te4 devices. Our work provides an efficient means for modulating topological quantum states and topological quantum phase transitions.",2107.03224v1 2021-07-22,Anomalous Transport in High-Mobility Superconducting SrTiO$_3$ Thin Films,"The study of subtle effects on transport in semiconductors requires high-quality epitaxial structures with low defect density. Using hybrid molecular beam epitaxy (MBE), SrTiO$_3$ films with low-temperature mobility exceeding 42,000 cm$^2$V$^{-1}$s$^{-1}$ at low carrier density of 3 x 10$^{17}$ cm$^{-3}$ were achieved. A sudden and sharp decrease in residual resistivity accompanied by an enhancement in the superconducting transition temperature were observed across the second Lifshitz transition (LT) where the third band becomes occupied, revealing dominant intra-band scattering. These films further revealed an anomalous behavior in the Hall carrier density as a consequence of the antiferrodistortive (AFD) transition and the temperature-dependence of the Hall scattering factor. Using hybrid MBE growth, phenomenological modeling, temperature-dependent transport measurements, and scanning superconducting quantum interference device imaging, we provide critical insights into the important role of inter- vs intra-band scattering and of AFD domain walls on normal-state and superconducting properties of SrTiO$_3$.",2107.10904v1 2021-09-27,Pressure-induced monotonic enhancement of Tc to over 30 K in the superconducting Pr0.82Sr0.18NiO2 thin films,"The successful synthesis of superconducting infinite-layer nickelate thin films with the highest Tc ~ 15 K has reignited great enthusiasms on this family of potential analogue to high-Tc cuprates. Pursuing a higher Tc is always an imperative task in studying a new superconducting material system. Here we report high-quality Pr0.82Sr0.18NiO2 thin films with Tconset ~ 17 K synthesized by carefully tuning the amount of CaH2 in the topological chemical reduction and the effect of pressure on its superconducting properties by measuring electrical resistivity under various pressures in a cubic anvil cell apparatus. We find that the onset temperature of the superconductivity, Tconset, can be enhanced monotonically from ~ 17 K at ambient pressure to ~ 31 K at 12.1 GPa without showing signatures of saturation upon increasing pressure. This encouraging result indicates that the Tc of infinite-layer nickelates superconductors still has room to go higher and it can be further boosted by applying higher pressures or strain engineering in the heterostructure films.",2109.12811v2 2021-10-26,Novel Lithium-Sulfur Polymer Battery Operating at Moderate Temperature,"A safe lithium-sulfur (Li-S) battery employs a composite polymer electrolyte based on a poly(ethylene glycol) dimethyl ether (PEGDME) solid at room temperature. The electrolyte membrane enables a stable and reversible Li-S electrochemical process already at 50{\deg}C, with low resistance at the electrode/electrolyte interphase and fast Li+ transport. The relatively low molecular weight of the PEGDME and the optimal membrane composition in terms of salts and ceramic allow a liquid-like Li-S conversion reaction by heating at moderately high temperature, still holding the solid-like polymer state of the cell. Therefore, the electrochemical reaction of the polymer Li-S cell is characterized by the typical dissolution of lithium polysulfides into the electrolyte medium during discharge and the subsequent deposition of sulfur at the electrode/electrolyte interphase during charge. On the other hand, the remarkable thermal stability of the composite polymer electrolyte (up to 300{\deg}C) suggests a lithium-metal battery with safety content significantly higher than that using the common, flammable liquid solutions. Hence, the Li-S polymer battery delivers at 50{\deg}C and 2 V a stable capacity approaching 700 mAhgS-1, with a steady-state coulombic efficiency of 98%. These results suggest a novel, alternative approach to achieve safe, high energy batteries with solid polymer configuration.",2110.13727v1 2021-11-30,Bosonic metal states in crystalline iron-based superconductors at the two-dimensional limit,"The nature of the anomalous metal, one of the quantum ground states of two-dimensional (2D) bosonic systems, remains a major puzzle even after several decades of study. Here, we report a systematic investigation on the transport properties of ultrathin crystalline FeSe films grown on SrTiO3 (STO) as well as the nanopatterned FeSe/STO, where the 2D high-temperature superconductivity is confined at the interface. Remarkably, the bosonic anomalous metal state emerges around 20 K, an exceptionally high temperature compared to all previous observations. Furthermore, a linear-in-temperature (T-linear) resistance with suppressed Hall coefficient below onset temperature for superconductivity is observed, indicating a bosonic strange metal. We give quantitative analysis for the bosonic anomalous metal state, based on the quantum dynamical property of vortices influenced by ohmic dissipation. This microscopic model pins down the origin of the intriguing anomalous state to the superconducting phase dynamics in both spatial and temporal domain. Our findings shed new light on the bosonic metal states in crystalline superconductors at the 2D limit.",2111.15488v2 2022-03-14,Large enhancement in thermal conductivity of solvent cast expanded-graphite/polyetherimide composites,"We demonstrate in this work, that expanded graphite (EG) can lead to a very large enhancement in thermal conductivity of polyetherimide-graphene and epoxy-graphene nanocomposites prepared via solvent casting technique. A k value of 6.56 Wm-1K-1 is achieved for 10 weight % composition sample, representing an enhancement of ~2770% over pristine polyetherimide (k ~ 0.23 Wm-1K-1). This extraordinary enhancement in thermal conductivity is shown to be due to a network of continuous graphene sheets over long length scales, resulting in low thermal contact resistance at bends/turns due to the graphene sheets being covalently bonded at such junctions. Solvent casting offers the advantage of preserving the porous structure of expanded graphite in the composite, resulting in the above highly thermally conductive interpenetrating network of graphene and polymer. Solvent casting also does not break down the expanded graphite particles, due to minimal forces involved, allowing for efficient heat transfer over long length scales, further enhancing overall composite thermal conductivity. Comparisons with a recently introduced effective medium model shows a very high value of predicted particle-particle interfacial conductance, providing evidence for efficient interfacial thermal transport in expanded graphite composites. Field Emission Environmental Scanning Electron Microscopy (FE-ESEM) is used to provide detailed understanding of interpenetrating graphene-polymer structure in the expanded graphite composite. These results open up novel avenues for achieving high thermal conductivity polymer composites.",2203.06828v1 2022-03-18,Thermoelectric transport properties of gapless pinned charge density waves,"Quantum strongly correlated matter exhibits properties which are not easily explainable in the conventional framework of Fermi liquids. Universal effective field theory tools are applicable in these cases regardless of the microscopic details of the quantum system, since they are based on symmetries. It is necessary, however, to construct these effective tools in full generality, avoiding restrictions coming from particular microscopic descriptions which may inadequately constrain the coefficients that enter in the effective theory. In this work we demonstrate on explicit examples how the novel hydrodynamic coefficients which have been recently reinstated in the effective theory of pinned charge density waves (CDW) can affect the phenomenology of the thermo-electric transport in strongly correlated quantum matter. Our examples, based on two classes of holographic models with pinned CDW, have microscopics which are conceptually different from Fermi liquids. Therefore, the above novel transport coefficients are nonzero, contrary to the conventional approach. We show how these coefficients allow to take into account the change of sign of the Seebeck coefficient and the low resistivity of the CDW phase of the cuprate high temperature superconductors, without referring to the effects of Fermi surface reconstruction.",2203.10038v2 2022-05-11,An mCherry biolaser based on microbubble cavity with ultra-low threshold,"Biolasers show considerable potential in the biomedical field. Fluorescent protein (FP) is a type of biomaterial with good luminescence efficiency that can be used as the luminescent gain medium in biolasers. Due to the higher cell/tissue permeability, lower cell phototoxicity, and relatively less background fluorescence than other fluorescent proteins, the red fluorescent protein is more suitable in biological applications. MCherry is the most extensively used high-quality red fluorescent protein because of its short maturation time and stable luminescence properties. In this study, using mCherry and microbubble cavity, we realize a highly stable mCherry fluorescent protein laser. The laser resonator achieves a quality factor of 10^8, which is the highest Q factor among the currently available FP lasers. Moreover, this laser exhibits low threshold of 286 fJ, which can effectively protect the luminescent material from being damaged by pump light. Such a threshold is the lowest in the FP lasers as per our knowledge. The prepared laser shows excellent stability in a wide pH range with good photobleaching resistance and can be stored at 4 degree for nearly a month. Also, the laser can serve as a high-sensitivity molecular concentration detector with mCherry as biomarker, owing to its lasing threshold behavior.",2205.05220v2 2022-07-01,Efficient and Scalable GaInAs Thermophotovoltaic Devices,"Thermophotovoltaics are promising solid-state energy converters for a variety of applications such as grid-scale energy storage, concentrating solar-thermal power, and waste heat recovery. Here, we report the design, fabrication, and testing of large area (0.8 cm$^2$), scalable, single junction 0.74-eV GaInAs thermophotovoltaic devices reaching an efficiency of 38.8$\pm$2.0% and an electrical power density of 3.78 W/cm$^2$ at an emitter temperature of 1850{\deg}C. Reaching such a high emitter temperature and power density without sacrificing efficiency is a direct result of combining good spectral management with a highly optimized cell architecture, excellent material quality, and very low series resistance. Importantly, fabrication of 12 high-performing devices on a two-inch wafer is shown to be repeatable, and the cell design can be readily transferred to commercial epitaxy on even larger wafers. Further improvements in efficiency can be obtained by using a multijunction architecture, and early results for a two-junction 0.84-eV GaInPAs / 0.74-eV GaInAs device illustrate this promise.",2207.00565v1 2022-07-12,Non-destructive Depth-Resolved Characterization of Residual Strain Fields in High Electron Mobility Transistors using Differential Aperture X-ray Microscopy,"Localized residual stress and elastic strain concentrations in microelectronic devices often affect the electronic performance, resistance to thermomechanical damage, and, likely, radiation tolerance. A primary challenge for characterization of these concentrations is that they exist over sub-$\mu$m length-scales, precluding their characterization by more traditional residual stress measurement techniques. Here we demonstrate the use of synchrotron X-ray -based differential aperture X-ray microscopy (DAXM) as a viable, non-destructive means to characterize these stress and strain concentrations in a depth-resolved manner. DAXM is used to map two-dimensional strain fields between source and drain in a gallium nitride (GaN) layer within high electron mobility transistors (HEMTs) with sub-$\mu$m spatial resolution. Strain fields at various positions in both pristine and irradiated HEMT specimens are presented in addition to a preliminary stress analysis to estimate the distribution of various stress components within the GaN layer. $\gamma$-irradiation is found to significantly reduce the lattice plane spacing in the GaN along the sample normal direction which is attributed to radiation damage in transistor components bonded to the GaN during irradiation.",2207.05789v2 2022-08-10,Synthesis of Superconducting Phase of La$_{0.5}$Ce$_{0.5}$H$_{10}$ at High Pressures,"Clathrate hydride \emph{Fm}\={3}\emph{m}-LaH$_{10}$ has been proven as the most extraordinary superconductor with the critical temperature $T_c$ above 250 K upon compression of hundreds of GPa in recent years. A general hope is to reduce the stabilization pressure and maintain the high $T_c$ value of the specific phase in LaH$_{10}$. However, strong structural instability distorts \emph{Fm}\={3}\emph{m} structure and leads to a rapid decrease of $T_c$ at low pressures. Here, we investigate the phase stability and superconducting behaviors of \emph{Fm}\={3}\emph{m}-LaH$_{10}$ with enhanced chemical pre-compression through partly replacing La by Ce atoms from both experiments and calculations. For explicitly characterizing the synthesized hydride, we choose lanthanum-cerium alloy with stoichiometry composition of 1:1. X-ray diffraction and Raman scattering measurements reveal the stabilization of \emph{Fm}\={3}\emph{m}-La$_{0.5}$Ce$_{0.5}$H$_{10}$ in the pressure range of 140-160 GPa. Superconductivity with $T_c$ of 175$\pm$2 K at 155 GPa is confirmed with the observation of the zero-resistivity state and supported by the theoretical calculations. These findings provide applicability in the future explorations for a large variety of hydrogen-rich hydrides.",2208.05199v1 2022-09-12,Emergent magnetic states and tunable exchange bias at all 3d nitride heterointerfaces,"Interfacial magnetism stimulates the discovery of giant magnetoresistance and spin-orbital coupling across the heterointerfaces, facilitating the intimate correlation between spin transport and complex magnetic structures. Over decades, functional heterointerfaces composed of nitrides are seldomly explored due to the difficulty in synthesizing high-quality and correct composition nitride films. Here we report the fabrication of single-crystalline ferromagnetic Fe3N thin films with precisely controlled thickness. As film thickness decreasing, the magnetization deteriorates dramatically, and electronic state transits from metallic to insulating. Strikingly, the high-temperature ferromagnetism maintains in a Fe3N layer with a thickness down to 2 u. c. (~ 8 {\AA}). The magnetoresistance exhibits a strong in-plane anisotropy and meanwhile the anomalous Hall resistance reserves its sign when Fe3N layer thickness exceeds 5 u. c. Furthermore, we observe a sizable exchange bias at the interfaces between a ferromagnetic Fe3N and an antiferromagnetic CrN. The exchange bias field and saturation moment strongly depend on the controllable bending curvature using cylinder diameter engineering (CDE) technique, implying the tunable magnetic states under lattice deformation. This work provides a guideline for exploring functional nitride films and applying their interfacial phenomena for innovative perspectives towards the practical applications.",2209.05209v1 2022-11-02,Tunable Rapid Electron Transport in Titanium Oxide Thin Films,"Rapid electron transport in the quantum well triggers many novel physical phenomena and becomes a critical point for the high-speed electronics. Here, we found electrical properties of the titanium oxide changed from semiconducting to metallic as the degree of oxidation decreased and Schottky quantum well was formed at the interface. We take the asymmetry interface electron scattering effect into consideration when studying the electrical transport properties of the multilayer thin films. A novel physical conductivity model for the multilayer thin films was developed. We found electron would be transferred from the low-mobility semiconducting and metallic conductive channels to the high-mobility Schottky quantum well conductive channel with an in-plane applied electric field. Electron concentration and mobility of the forming 2DEG in the Schottky quantum well could be tuned thus the nano-devices exhibited non-linear voltage-current curves. The differential resistivity of the nano-devices could decrease by two orders with increasing electric field at room temperature. Weak electron localization of electrons has been experimentally observed in our nano-devices at low temperature, which further demonstrated the existence of 2DEG in the Schottky quantum well. Our work will provide us new physics about the rapid electron transport in the multilayer thin films, and bring novel functional devices for the modern microelectronic industry.",2211.01162v1 2023-03-06,A Miniaturised Camera-based Multi-Modal Tactile Sensor,"In conjunction with huge recent progress in camera and computer vision technology, camera-based sensors have increasingly shown considerable promise in relation to tactile sensing. In comparison to competing technologies (be they resistive, capacitive or magnetic based), they offer super-high-resolution, while suffering from fewer wiring problems. The human tactile system is composed of various types of mechanoreceptors, each able to perceive and process distinct information such as force, pressure, texture, etc. Camera-based tactile sensors such as GelSight mainly focus on high-resolution geometric sensing on a flat surface, and their force measurement capabilities are limited by the hysteresis and non-linearity of the silicone material. In this paper, we present a miniaturised dome-shaped camera-based tactile sensor that allows accurate force and tactile sensing in a single coherent system. The key novelty of the sensor design is as follows. First, we demonstrate how to build a smooth silicone hemispheric sensing medium with uniform markers on its curved surface. Second, we enhance the illumination of the rounded silicone with diffused LEDs. Third, we construct a force-sensitive mechanical structure in a compact form factor with usage of springs to accurately perceive forces. Our multi-modal sensor is able to acquire tactile information from multi-axis forces, local force distribution, and contact geometry, all in real-time. We apply an end-to-end deep learning method to process all the information.",2303.03093v1 2023-03-15,Rare observation of spin-gapless semiconducting characteristics and related band topology of quaternary Heusler alloy CoFeMnSn,"In this paper, we report the theoretical investigation and experimental realization of a new spin-gapless semiconductor (SGSs) compound CoFeMnSn belonging to the family of quaternary Heusler alloys. Through the use of several ground-state energy calculations, the most stable structure has been identified. Calculations of the spin-polarized band structure in optimized structure's reveals the SGS nature of the compound. The compound form in an ordered crystal structure and exhibit a high ferromagnetic transition temperature (T$_{\rm C}$ = 560 K), making the material excellent for room temperature applications. Adherence of saturation magnetization to the Slater-Pauling rule, together with the nearly temperature-independent resistivity, conductivity, and carrier concentration of the compound in the temperature regime 5$-$300 K along with the low value of anomalous Hall conductivity (AHC) further confirms the SGS nature. Theoretical calculations also reveal the robustness of the SGS state due to lattice contraction and one can obtain a high value of intrinsic AHC using hole doping. Combined SGS and topological properties of the compound make CoFeMnSn suitable for spintronics and magneto-electronics devices.",2303.08589v2 2023-04-11,"Effects of equivalent composition on superconducting properties of high-entropy REOBiS$_2$ (RE = La, Ce, Pr, Nd, Sm, Gd) single crystals","Superconductors are influenced by high-entropy alloys (HEAs); these have been investigated in various functional materials. REOBiS$_2$ (RE = La, Ce, Pr, Nd, Sm, and Gd in different combinations) single crystals with HEAs at the RE-site were successfully grown using the flux method. The obtained crystals were plate-shaped (1 mm$^2$) with a well-developed c-plane. Ce was present in both trivalent (Ce$^{3+}$) and tetravalent (Ce$^{4+}$) electronic configurations; the concentration of Ce$^{4+}$ at the RE-site was approximately 10 at% in all single crystals. The single crystals showed superconducting transition temperature with zero resistivity within 1.2-4.2 K. The superconducting transition temperature, superconducting anisotropy, electronic specific heat coefficient, and Debye temperature of the crystals were not correlated with the mixed entropy at the RE-site. Except for the electronic specific heat coefficient, the variation of these parameters as a function of mixed entropy showed different trends for equivalent and non-equivalent RE element compositions. Thus, the configuration of RE elements influences the superconducting properties of REOBiS$_2$ single crystals, alluding to a method of modulating transition temperatures.",2304.04993v1 2023-06-21,An Analytical Model to Quantify the Local Lattice Distortion of Refractory High Entropy Alloys,"Local lattice distortion (LLD) of high entropy alloys (HEAs) especially refractory HEAs, which is different from one lattice site to another, determines the mechanical properties of HEAs such as yield strength and radiation resistance, and is crucial to modulating catalytic activity of HEAs via the atomic strain. In particular, this site-to-site LLD is strongly coupled with the short-range order (SRO) of HEAs. Therefore it is essential to reveal the physical picture of LLD. However, the random distribution of multi-principal constituents of HEAs prohibits the understanding of LLD, including the determinants of LLD and their coupling rules. Herein, we build the first analytical model to realize the site-to-site prediction of LLD in refractory HEAs, by using the neighbor number ratio of central atoms, the central-atom radii, the standard deviation of constituent radii and the constituent number, which demonstrates that LLD surprisingly exhibits a similar mechanism as the relaxation of metal surfaces. The involved parameters depend only on the radii of constituents and are readily accessible. Moreover, our scheme determines not only LLD but also the average lattice distortion, which enables us to predict the phase stability and yield strength of HEAs. These results build a novel physical picture of LLD, in particular the quantitative relationship between LLD and SRO, which lay a solid foundation for the further target-oriented design of HEAs.",2306.11959v1 2023-06-28,High-Q trenched aluminum coplanar resonators with an ultrasonic edge microcutting for superconducting quantum devices,"Dielectric losses are one of the key factors limiting the coherence of superconducting qubits. The impact of materials and fabrication steps on dielectric losses can be evaluated using coplanar waveguide (CPW) microwave resonators. Here, we report on superconducting CPW microwave resonators with internal quality factors systematically exceeding 5x106 at high powers and 2x106 (with the best value of 4.4x106) at low power. Such performance is demonstrated for 100-nm-thick aluminum resonators with 7-10.5 um center trace on high-resistivity silicon substrates commonly used in quantum Josephson junction circuits. We investigate internal quality factors of the resonators with both dry and wet aluminum etching, as well as deep and isotropic reactive ion etching of silicon substrate. Josephson junction compatible CPW resonators fabrication process with both airbridges and silicon substrate etching is proposed. Finally, we demonstrate the effect of airbridges positions and extra process steps on the overall dielectric losses. The best quality fa ctors are obtained for the wet etched aluminum resonators and isotropically removed substrate with the proposed ultrasonic metal edge microcutting.",2306.16301v1 2023-10-05,"Liquid Cooling System for a High Power, Medium Frequency, and Medium Voltage Isolated Power Converter","Power electronics systems, widely used in various applications such as industrial automation, electric cars, and renewable energy, have the primary function of converting and controlling electrical power to the desired type of load. Despite their reliability and efficiency, power losses in these systems generate significant heat that must be dissipated to maintain performance and prevent damage. Cooling systems play a crucial role in ensuring safe operating temperatures for system components. Air and liquid cooling are the leading technologies used in the power electronics world. Air cooling is simple and cost-effective but is limited by ambient temperature and component thermal resistance. While more efficient, liquid cooling requires more maintenance and has higher upfront costs. Water-cooling systems have become famous for regulating thermal loads as they can effectively remove heat from localized high-temperature areas, such as the challenging hotspots in power electronics systems. In addition to designing a cooling system for a power electronic system, this study investigated the impact of three major parameters; cold plate material, channel shape/size, and coolant inlet velocity. The research examined and analyzed these factors and their trade-off analysis to obtain cooling system design and optimization insights. This study might improve power electronics system performance, reliability, and durability by improving heat dissipation and thermal management.",2310.03577v1 2023-10-19,Detailed and high-throughput measurement of composition dependence of magnetoresistance and spin-transfer torque using a composition-gradient film: application to Co$_{x}$Fe$_{1-x}$ (0 $\le$ $\textit{x}$ $\le$ 1) system,"We develop a high-throughput method for measuring the composition dependence of magnetoresistance (MR) and spin-transfer-torque (STT) effects in current-perpendicular-to-plane giant magnetoresistance (CPP-GMR) devices and report its application to the CoFe system. The method is based on the use of composition-gradient films deposited by combinatorial sputtering. This structure allows the fabrication of devices with different compositions on a single substrate, drastically enhancing the throughput in investigating composition dependence. We fabricated CPP-GMR devices on a single GMR film consisting of a Co$_{x}$Fe$_{1-x}$ (0 $\le$ $\textit{x}$ $\le$ 1) composition-gradient layer, a Cu spacer layer, and a NiFe layer. The MR ratio obtained from resistance-field measurements exhibited the maximum in the broad Co concentration range of 0.3 $\le$ $\textit{x}$ $\le$ 0.65. In addition, the STT efficiency was estimated from the current to induce magnetization reversal of the NiFe layer by spin injection from the Co$_{x}$Fe$_{1-x}$ layer. The STT efficiency was also the highest around the same Co concentration range as for the MR ratio, and this correlation was theoretically explained by the change in the spin polarization of the Co$_{x}$Fe$_{1-x}$ layer. The results revealed the Co$_{x}$Fe$_{1-x}$ composition range suitable for spintronic applications, demonstrating the advantages of the developed method.",2310.12434v1 2023-11-25,Our Dark Matter Stopping in the Earth,"We have worked for some time on a model for dark matter, in which dark matter consists of small bubbles of a new speculated type of vacuum, which are pumped up by some ordinary matter such as diamond, so as to resist the pressure of the domain wall separating the two vacua. Here we put forward thoughts on, how such macroscopic pearls would have their surrounding dust cleaned off passing through the atmosphere and the Earth, and what their distribution would be as a function of the depth of their stopping point and the distribution of the radiation emitted from them. In our model we assume that they radiate 3.5 keV electrons and photons, after having been excited during their passage into the Earth. The purpose of such an estimation of the radiation distribution is to explain the truly mysterious fact that, among all the underground experiments seeking dark matter colliding with the Earth material, only the DAMA-LIBRA experiment has seen any evidence of dark matter. This is an experiment based on solid NaI scintillators and is rather deep at 1400 m. It is our point that we can arrange the main radiation to appear in the relatively deep DAMA- LIBRA site, and explain that the dark matter pearls cannot stop in a fluid, such as xenon in the xenon based experiments.",2311.14996v1 2023-11-27,Tailoring the Opto-Electronic Properties of Oxide-Metal-Oxide Transparent Electrode Using Cu Seed Layer,"The oxide-metal-oxide architecture is a promising approach for the development of the high-performance indium-free transparent electrode (TE), which is a key component of various optoelectronic applications such as solar cells, organic LEDs, and touchscreen panels. Here in this work, we have shown high-performance TE consisting of TiO2/Ag/TiO2 (TAT), with the incorporation of a copper seed layer. The seed layer increases the wettability and improves the adhesion of deposited Ag film on the bottom TiO2 layer. Before the experimental realization, optical modeling is performed by using MATLAB code based on the transfer matrix method. The optimum thickness obtained from the simulation is 30 nm for both undercoat and overcoat TiO2 with the average transmittance in the visible region >85% with the Ag thickness of 9nm. With inputs from the optical modeling, TEs were experimentally realized with and without the Cu seed layer. It has been found that the TE with an additional sputtered Cu (1 nm) seed layer is essential for the smooth growth of silver film and shows better electro-optical performance (sheet resistance < 10 and average transmittance in the visible spectral range > 80%) than TAT-TE without any seed layer. The electro-optical and morphological properties of the TiO2/Cu/Ag/TiO2 structure make it suitable for optoelectronic applications.",2311.15535v2 2023-11-30,Vanishing of the anomalous Hall effect and enhanced carrier mobility in the spin-gapless ferromagnetic Mn2CoGa1-xAlx alloys,"Spin gapless semiconductor (SGS) has attracted long attention since its theoretical prediction, while concrete experimental hints are still lack in the relevant Heusler alloys. Here in this work, by preparing the series alloys of Mn2CoGa1-xAlx (x=0, 0.25, 0.5, 0.75 and 1), we identified the vanishing of anomalous Hall effect in the ferromagnetic Mn2CoGa (or x=0.25) alloy in a wide temperature interval, accompanying with growing contribution from the ordinary Hall effect. As a result, comparatively low carrier density (1020 cm-3) and high carrier mobility (150 cm2/Vs) are obtained in Mn2CoGa (or x=0.25) alloy in the temperature range of 10-200K. These also lead to a large dip in the related magnetoresistance at low fields. While in high Al content, despite the magnetization behavior is not altered significantly, the Hall resistivity is instead dominated by the anomalous one, just analogous to that widely reported in Mn2CoAl. The distinct electrical transport behavior of x=0 and x=0.75 (or 1) is presently understood by their possible different scattering mechanism of the anomalous Hall effect due to the differences in atomic order and conductivity. Our work can expand the existing understanding of the SGS properties and offer a better SGS candidate with higher carrier mobility that can facilitate the application in the spin-injected related devices.",2311.18335v1 2024-01-31,Electrical 180o switching of Néel vector in spin-splitting antiferromagnet,"Antiferromagnetic spintronics have attracted wide attention due to its great potential in constructing ultra-dense and ultra-fast antiferromagnetic memory that suits modern high-performance information technology. The electrical 180o switching of N\'eel vector is a long-term goal for developing electrical-controllable antiferromagnetic memory with opposite N\'eel vectors as binary ""0"" and ""1"". However, the state-of-art antiferromagnetic switching mechanisms have long been limited for 90o or 120o switching of N\'eel vector, which unavoidably require multiple writing channels that contradicts ultra-dense integration. Here, we propose a deterministic switching mechanism based on spin-orbit torque with asymmetric energy barrier, and experimentally achieve electrical 180o switching of spin-splitting antiferromagnet Mn5Si3. Such a 180o switching is read out by the N\'eel vector-induced anomalous Hall effect. Based on our writing and readout methods, we fabricate an antiferromagnet device with electrical-controllable high and low resistance states that accomplishes robust write and read cycles. Besides fundamental advance, our work promotes practical spin-splitting antiferromagnetic devices based on spin-splitting antiferromagnet.",2401.17608v1 2024-02-29,Controllable suppression of the unconventional superconductivity in bulk and thin-film Sr$_{2}$RuO$_{4}$ via high-energy electron irradiation,"In bulk Sr$_{2}$RuO$_{4}$, the strong sensitivity of the superconducting transition temperature $T_{\text{c}}$ to nonmagnetic impurities provides robust evidence for a superconducting order parameter that changes sign around the Fermi surface. In superconducting epitaxial thin-film Sr$_{2}$RuO$_{4}$, the relationship between $T_{\text{c}}$ and the residual resistivity $\rho_0$, which in bulk samples is taken to be a proxy for the low-temperature elastic scattering rate, is far less clear. Using high-energy electron irradiation to controllably introduce point disorder into bulk single-crystal and thin-film Sr$_{2}$RuO$_{4}$, we show that $T_{\text{c}}$ is suppressed in both systems at nearly identical rates. This suggests that part of $\rho_0$ in films comes from defects that do not contribute to superconducting pairbreaking, and establishes a quantitative link between the superconductivity of bulk and thin-film samples.",2402.19454v1 2017-07-09,Ultrafast Epitaxial Growth of Metre-Sized Single-Crystal Graphene on Industrial Cu Foil,"A foundation of the modern technology that uses single-crystal silicon has been the growth of high-quality single-crystal Si ingots with diameters up to 12 inches or larger. For many applications of graphene, large-area high-quality (ideally of single-crystal) material will be enabling. Since the first growth on copper foil a decade ago, inch-sized single-crystal graphene has been achieved. We present here the growth, in 20 minutes, of a graphene film of 5 x 50 cm2 dimension with > 99% ultra-highly oriented grains. This growth was achieved by: (i) synthesis of sub-metre-sized single-crystal Cu(111) foil as substrate; (ii) epitaxial growth of graphene islands on the Cu(111) surface; (iii) seamless merging of such graphene islands into a graphene film with high single crystallinity and (iv) the ultrafast growth of graphene film. These achievements were realized by a temperature-driven annealing technique to produce single-crystal Cu(111) from industrial polycrystalline Cu foil and the marvellous effects of a continuous oxygen supply from an adjacent oxide. The as-synthesized graphene film, with very few misoriented grains (if any), has a mobility up to ~ 23,000 cm2V-1s-1 at 4 K and room temperature sheet resistance of ~ 230 ohm/square. It is very likely that this approach can be scaled up to achieve exceptionally large and high-quality graphene films with single crystallinity, and thus realize various industrial-level applications at a low cost.",1707.02512v1 2020-06-04,Thermal conductivity of amorphous and crystalline GeTe thin film at high temperature: Experimental and theoretical study,"Thermal transport properties bear a pivotal role in influencing the performance of phase change memory (PCM) devices, in which the PCM operation involves fast and reversible phase change between amorphous and crystalline phases. In this paper, we present a systematic experimental and theoretical study on the thermal conductivity of GeTe at high temperatures involving fast change from amorphous to crystalline phase upon heating. Modulated photothermal radiometry (MPTR) is used to experimentally determine thermal conductivity of GeTe at high temperatures in both amorphous and crystalline phases. Thermal boundary resistances are accurately taken into account for experimental consideration. To develop a concrete understanding of the underlying physical mechanism, rigorous and in-depth theoretical exercises are carried out. For this, first-principles density functional methods and linearized Boltzmann transport equations (LBTE) are employed using both direct and relaxation time based approach (RTA) and compared with that of the phenomenological Slack model. The amorphous phase experimental data has been described using the minimal thermal conductivity model with sufficient precision. The theoretical estimation involving direct solution and RTA method are found to retrieve well the trend of the experimental thermal conductivity for crystalline GeTe at high temperatures despite being slightly overestimated and underestimated, respectively, compared to the experimental data. A rough estimate of vacancy contribution has been found to modify the direct solution in such a way that it agrees excellently with the experiment. Umklapp scattering has been determined as the significant phonon-phonon scattering process. Umklapp scattering parameter has been identified for GeTe for the whole temperature range which can uniquely determine and compare Umklapp scattering processes for different materials",2006.02625v1 2021-08-31,Toward 100% Spin-Orbit Torque Efficiency with High Spin-Orbital Hall Conductivity Pt-Cr Alloys,"5d transition metal Pt is the canonical spin Hall material for efficient generation of spin-orbit torques (SOTs) in Pt/ferromagnetic layer (FM) heterostructures. However, for a long while with tremendous engineering endeavors, the damping-like SOT efficiencies (${\xi}_{DL}$) of Pt and Pt alloys have still been limited to ${\xi}_{DL}$<0.5. Here we present that with proper alloying elements, particularly 3d transition metals V and Cr, a high spin-orbital Hall conductivity (${\sigma}_{SH}{\sim}6.5{\times}10^{5}({\hbar}/2e){\Omega}^{-1}{\cdot} m^{-1}$) can be developed. Especially for the Cr-doped case, an extremely high ${\xi}_{DL}{\sim}0.9$ in a Pt$_{0.69}$Cr$_{0.31}$/Co device can be achieved with a moderate Pt$_{0.69}$Cr$_{0.31}$ resistivity of ${\rho}_{xx}{\sim}133 {\mu}{\Omega}{\cdot}cm$. A low critical SOT-driven switching current density of $J_{c}{\sim}3.2{\times}10^{6} A{\cdot}cm^{-2}$ is also demonstrated. The damping constant (${\alpha}$) of Pt$_{0.69}$Cr$_{0.31}$/FM structure is also found to be reduced to 0.052 from the pure Pt/FM case of 0.078. The overall high ${\sigma}_{SH}$, giant ${\xi}_{DL}$, moderate ${\rho}_{xx}$, and reduced ${\alpha}$ of such a Pt-Cr/FM heterostructure makes it promising for versatile extremely low power consumption SOT memory applications.",2108.13857v3 2024-01-05,Signatures of room-temperature superconductivity emerging in two-dimensional domains within the new Bi/Pb-based ceramic cuprate superconductors at ambient pressure,"We predict the possibility of realizing room-temperature superconductivity in different 2D domains within the ceramic high-Tc cuprates at ambient pressure and experimentally confirm this prediction of 2D room-temperature superconductivity in the newly derived Bi/Pb-based ceramic cuprates containing many grain boundaries, interfaces and multiplate blocks. We argue that, in these high-Tc materials, besides bulk superconductivity in 3D domains there is also strongly enhanced 2D superconductivity emerging in the 3D-2D crossover region well above the superconducting transition temperature Tc. We study the possibility of the existence of distinct 3D and 2D superconducting phases in high-Tc ceramic cuprates, in which the unconventional Cooper pairs behave like bosons and condense below certain critical temperatures into 3D and 2D Bose superfluids in 3D and 2D domains. We show that the superconducting transition temperature in 2D domains is much higher than in 3D domains and can reach up to room temperature. We report signatures of room-temperature superconductivity occurring at different grain boundaries and 3D/2D interfaces and in multiplate blocks within the ceramic superconductors, synthesized by using the new melt technology in a large solar furnace. The samples of these materials synthesized under the influence of concentrated solar energy have the bulk Tc values ranging from 100 K to about 140 K and the more higher superconducting transition temperatures, possibly even as high as room temperature in the 3D-2D crossover region. The remnant 2D superconductivity in newly derived Bi/Pb-based ceramic cuprate superconductors is observed at temperatures 200-300 K well above the bulk Tc and the onset of room-temperature superconductivity is evidenced by the observations of a sharp step-like drop in the resistance and a well-detectable partial Meissner effect at around 300 K and ambient pressure.",2401.02642v1 2024-04-17,On-liquid-gallium surface synthesis of ultra-smooth conductive metal-organic framework thin films,"Conductive metal-organic frameworks (MOFs) are emerging electroactive materials for (opto-)electronics. However, it remains a great challenge to achieve reliable MOF-based devices via the existing synthesis methods that are compatible with the complementary metal-oxide-semiconductor technology, as the surface roughness of thus-far synthetic MOF films or pellets is rather high for efficient electrode contact. Here, we develop an on-liquid-gallium surface synthesis (OLGSS) strategy under chemical vapor deposition (CVD) conditions for the controlled growth of two-dimensional conjugated MOF (2D c-MOF) thin films with ten-fold improvement of surface flatness (surface roughness can reach as low as ~2 {\AA}) compared with MOF films grown by the traditional methods. Supported by theoretical modeling, we unveil a layer-by-layer CVD growth mode for constructing flattening surfaces, that is triggered by the high adhesion energy between gallium (Ga) and planar aromatic ligands. We further demonstrate the generality of the as-proposed OLGSS strategy by reproducing such a flat surface over nine different 2D c-MOF films with variable thicknesses (~2 to 208 nm) and large lateral sizes (over 1 cm2). The resultant ultra-smooth 2D c-MOF films enable the formation of high-quality electrical contacts with gold (Au) electrodes, leading to a reduction of contact resistance by over ten orders of magnitude compared to the traditional uneven MOF films. Furthermore, due to the efficient interfacial interaction benifited from the high-quality contacts, the prepared van der Waals heterostructure (vdWH) of OLGSS c-MOF and MoS2 exhibits intriguing photoluminescence (PL) enhancement, PL peak shift and large work function modulation. The establishment of the reliable OLGSS method provides the chances to push the development of MOF electronics and the construction of multicomponent MOF-based heterostructure materials.",2404.15357v1 2009-01-08,Transport properties of Layer-Antiferromagnet CuCrS2: A possible thermoelectric material,"The electrical, thermal conductivity and Seebeck coefficient of the quenched, annealed and slowly cooled phases of the layer compound CuCrS2 have been reported between 15K to 300K. We also confirm the antiferromagnetic transition at 40K in them by our magnetic measurements between 2K and 300K. The crystal flakes show a minimum around 100K in their in-plane resistance behavior. For the polycrystalline pellets the resistivity depends on their flaky texture and it attains at most 10 to 20 times of the room temperature value at the lowest temperature of measurement. The temperature dependence is complex and no definite activation energy of electronic conduction can be discerned. We find that the Seebeck coefficient is between 200-450 microV/K and is unusually large for the observed resistivity values of between 5-100 mOhm-cm at room temperature. The figure of merit ZT for the thermoelectric application is 2.3 for our quenched phases, which is much larger than 1 for useful materials. The thermal conductivity K is mostly due to lattice conduction and is reduced by the disorder in Cu- occupancy in our quenched phase. A dramatic reduction of electrical and thermal conductivity is found as the antiferromagnetic transition is approached from the paramagnetic region, and K subsequently rises in the ordered phase. We discuss the transport properties as being similar to a doped Kondo-insulator.",0901.0977v2 2009-06-29,A novel wear-resistant magnetic thin film material based on a $Ti_{1-x}Fe_xC_{1-y}$ nanocomposite alloy,"In this study we report on the film growth and characterization of thin (approximately 50 nm thick) Ti-Fe-C films deposited on amorphous quartz. The experimental studies have been complemented by first principles density functional theory (DFT) calculations. Upon annealing of as-prepared films, the composition of the metastable Ti-Fe-C film changes. An iron-rich phase is first formed close to the film surface, but with increasing annealing time this phase is gradually displaced toward the film-substrate interface where its position stabilizes. Both the magnetic ordering temperature and the saturation magnetization changes significantly upon annealing. The DFT calculations show that the critical temperature and the magnetic moment both increase with increasing Fe and C-vacancy concentration. The formation of the metastable iron-rich Ti-Fe-C compound is reflected in the strong increase of the magnetic ordering temperature. Eventually, after enough annealing time ($\geq 10$ minutes), nano-crystalline $\alpha$-Fe starts to precipitate and the amount and size of these precipitates can be controlled by the annealing procedure; after 20 minutes of annealing, the experimental results indicate a nano-crystalline iron-film embedded in a wear resistant TiC compound. This conclusion is further supported by transmission electron microscopy studies on epitaxial Ti-Fe-C films deposited on single crystalline MgO substrates where, upon annealing, an iron film embedded in TiC is formed. Our results suggest that annealing of metastable Ti-Fe-C films can be used as an efficient way of creating a wear-resistant magnetic thin film material.",0906.5386v1 2010-11-25,Resistive transition in disordered superconductors with varying intergrain coupling,"The effect of disorder is investigated in granular superconductive materials with strong and weak links. The transition is controlled by the interplay of the \emph{tunneling} $g$ and \emph{intragrain} $g_{intr}$ conductances, which depend on the strength of the intergrain coupling. For $g \ll g_{intr}$, the transition involves first the grain boundary, while for $g \sim g_{intr}$ the transition occurs into the whole grain. The different intergrain coupling is considered by modelling the superconducting material as a disordered network of Josephson junctions. Numerical simulations show that on increasing the disorder, the resistive transition occurs for lower temperatures and the curve broadens. These features are enhanced in disordered superconductors with strong links. The different behaviour is further checked by estimating the average network resistance for weak and strong links in the framework of the effective medium approximation theory. These results may be relevant to shed light on long standing puzzles as: (i) enhancement of the superconducting transition temperature of many metals in the granular states; (ii) suppression of superconductivity in homogeneously disordered films compared to standard granular systems close to the metal-insulator transition; (iii) enhanced degradation of superconductivity by doping and impurities in strongly linked materials, such as magnesium diboride, compared to weakly-linked superconductors, such as cuprates.",1011.5607v1 2015-10-23,Consequences of breaking time reversal symmetry in LaSb: a resistivity plateau and extreme magnetoresistance,"Time reversal symmetry (TRS) protects the metallic surface modes of topological insulators (TIs). The transport signature of robust metallic surface modes of TIs is a plateau that arrests the exponential divergence of the insulating bulk with decreasing temperature. This universal behavior is observed in all TI candidates ranging from Bi2Te2Se to SmB6. Recently, several topological semimetals (TSMs) have been found that exhibit extreme magnetoresistance (XMR) and TI universal resistivity behavior revealed only when breaking TRS, a regime where TIs theoretically cease to exist. Among these new materials, TaAs and NbP are nominated for Weyl semimetal due to their lack of inversion symmetry, Cd3As2 is nominated for Dirac semimetal due to its linear band crossing at the Fermi level, and WTe2 is nominated for resonant compensated semimetal due to its perfect electron-hole symmetry. Here we introduce LaSb, a simple rock-salt structure material without broken inversion symmetry, without perfect linear band crossing, and without perfect electron-hole symmetry. Yet LaSb portrays all the exotic field induced behaviors of the aforementioned semimetals in an archetypal fashion. It shows (a) the universal TI resistivity with a plateau at 15 K, revealed by a magnetic field, (b) ultrahigh mobility of carriers in the plateau region, (c) quantum oscillations with a non-trivial Berry phase, and (d) XMR of about one million percent at 9 tesla rivaled only by WTe2 and NbP. Due to its dramatic simplicity, LaSb is the ideal model system to formulate a theoretical understanding of the exotic consequences of breaking TRS in TSMs.",1510.06931v1 2015-11-30,Electrical transport in nano-thick ZrTe$_5$ sheets: from three to two dimensions,"ZrTe$_5$ is a newly discovered topological material. Shortly after a single layer ZrTe$_5$ had been predicted to be a two-dimensional topological insulator, a handful of experiments have been carried out on bulk ZrTe$_5$ crystals, which however suggest that its bulk form may be a three-dimensional topological Dirac semimetal. We report the first transport study on ultra thin ZrTe$_5$ flakes down to 10 nm. A significant modulation of the characteristic resistivity maximum in the temperature dependence by thickness has been observed. Remarkably, the metallic behavior, occurring only below about 150 K in bulk, persists to over 320 K for flakes less than 20 nm thick. Furthermore, the resistivity maximum can be greatly tuned by ionic gating. Combined with the Hall resistance, we identify contributions from a semiconducting and a semimetallic bands. The enhancement of the metallic state in thin flakes are consequence of shifting of the energy bands. Our results suggest that the band structure sensitively depends on the film thickness, which may explain the divergent experimental observations on bulk materials.",1511.09315v2 2016-06-08,Multi-orbital physics in lithium-molybdenum purple-bronze: going beyond paradigm,"We investigate the role of inter-orbital fluctuations in the low energy physics of a quasi-1D material - lithium molybdenum purple bronze (LMO). It is an exceptional material that may provide us a long sought realization of a Tomonaga-Luttinger liquid (TLL) physics, but its behaviour at temperatures of the order of $T^*\approx 30$K remains puzzling despite numerous efforts. Here we make a conjecture that the physics around $T^*$ is dominated by multi-orbital excitations. Their properties can be captured using an excitonic picture. Using this relatively simple model we compute fermionic Green's function in the presence of excitons. We find that the spectral function is broadened with a Gaussian and its temperature dependence acquires an extra $T^1$ factor. Both effects are in perfect agreement with experimental findings. We also compute the resistivity for temperatures above and below critical temperature $T_o$. We explain an upturn of the resistivity at 28K and interpret the suppression of this extra component of resistivity when a magnetic field is applied along the conducting axis. Furthermore, in the framework of our model, we qualitatively discuss and consistently explain other experimentally detected peculiarities of purple bronze: the breaking of Wiedmann-Franz law and the magnetochromatic behaviour.",1606.02687v3 2016-10-08,Enhancement of Impedance by Chromium Substitution and Correlation with DC Resistivity in Cobalt Ferrite,"Chromium substituted cobalt ferrite with grain size less than the single domain (approx. 70 nm) has been prepared by the sol-gel method. XRD analysis reveals that the samples crystallize to cubic symmetry with spacegroup number 227. Two transition temperatures (TD (approx. 450 K) and TM (approx. 600 K) have been observed from the impedance verses temperature measurement. TD increases with the increase in frequency due to dipole response to the frequency. TM is comparable with the para-ferrimagnetic transition temperature of cobalt ferrite, which is independent of frequency. This result is well supported by the temperature dependent DC conductivity measurement. The modified Debye relaxation could be explained the impedance spectra of CoFe2-xCrxO4. The grain and grain boundary effect on impedance spectroscopy has been observed from Cole-Cole analysis. The ac conductivity follows Arrhenius behavior at different frequencies. All the samples exhibit the negative temperature coefficient of resistance behavior which reveals the semiconducting behavior of the material. The Mott VRH model could explain the DC electrical conductivity. Both ac impedance and DC resistivity are well co-related each other to explain the electron transport properties in Cr substituted cobalt ferrite. The electrical transport properties could be explained by the electron hopping between different metal ions via oxygen in the material.",1610.02489v1 2018-08-08,The viscosities of partially molten materials undergoing diffusion creep,"Partially molten materials resist shearing and compaction. This resistance is described by a fourth-rank effective viscosity tensor. When the tensor is isotropic, two scalars determine the resistance: an effective shear and an effective bulk viscosity. Here, calculations are presented of the effective viscosity tensor during diffusion creep for a 2D tiling of hexagonal unit cells and a 3D tessellation of tetrakaidecahedrons (truncated octahedrons). The geometry of the melt is determined by assuming textural equilibrium. The viscosity tensor for the 2D tiling is isotropic, but that for the 3D tessellation is anisotropic. Two parameters control the effect of melt on the viscosity tensor: the porosity and the dihedral angle. Calculations for both Nabarro-Herring (volume diffusion) and Coble (surface diffusion) creep are presented. For Nabarro-Herring creep the bulk viscosity becomes singular as the porosity vanishes. This singularity is logarithmic, a weaker singularity than typically assumed in geodynamic models. The presence of a small amount of melt (0.1% porosity) causes the effective shear viscosity to approximately halve. For Coble creep, previous modelling work has argued that a very small amount of melt may lead to a substantial, factor of 5, drop in the shear viscosity. Here, a much smaller, factor of 1.4, drop is obtained for tetrakaidecahedrons. Owing to a Cauchy relation symmetry, the Coble creep bulk viscosity is a constant multiple of the shear viscosity when melt is present.",1808.02734v2 2019-01-14,Gate tunable giant anisotropic resistance in ultra-thin GaTe,"In crystals, the duplication of atoms often follows different periodicity along different directions. It thus gives rise to the so called anisotropy, which is usually even more pronounced in two dimensional (2D) materials due to the absence of $\textbf{z}$ dimension. Indeed, in the emerging 2D materials, electrical anisotropy has been one of the focuses in recent experimental efforts. However, key understandings of the in-plane anisotropic resistance in low-symmetry 2D materials, as well as demonstrations of model devices taking advantage of it, have proven difficult. Here, we show that, in few-layered semiconducting GaTe, electrical conductivity along $\textbf{x}$ and $\textbf{y}$ directions of the 2D crystal can be gate tuned from a ratio of less than one order to as large as 10$^{3}$. This effect is further demonstrated to yield an anisotropic memory resistor behaviour in ultra-thin GaTe, when equipped with an architecture of van der Waals floating gate. Our findings of gate tunable giant anisotropic resistance (GAR) effect pave the way for potential applications in nano-electronics such as multifunctional directional memories in the 2D limit.",1901.04262v1 2020-01-27,Graphene-based Nanoscale version of da Vinci's Reciprocal Structures,"A reciprocal structure (RS) is a mechanical resistant structure formed by a set of self-supporting elements satisfying certain conditions of structural reciprocity (SR) . The first condition is that each element of the structure has to support and be supported by the others. The second condition is that these functions cannot occur in the same part of the element. These two properties make beams and two-dimensional materials very much appropriate to build RSs. Commonly seen in floors or roofs, SR is also present in art, religious symbols and decorative objects. Da Vinci has drawn several examples of such RSs. Here, we propose a simple nano version of a da Vinci's RS based on graphene nanoribbons. The stability and resistance against mechanical impacts (ballistic projectile) were investigated through fully atomistic molecular dynamics (MD) simulations. We considered structures with three and four joins with and without RS topologies. Our MD results showed that structures with RS topologies are more impact resistant than those without SR, despite the fact that the used graphene nanoribbons are highly pliable. We discuss these results in terms of the number of joins, energy absorption and stress on the structures. We discuss possible applications in nanoengineering.",2001.10027v2 2021-05-21,Vanadium Dioxide Thin Films Synthesized Using Low Thermal Budget Atmospheric Oxidation,"Vanadium dioxide is a complex oxide material, which shows large resistivity and optical reflectance change while transitioning from the insulator to metal phase at ~68 {\deg}C. In this work, we use a modified atmospheric thermal oxidation method to oxidize RF-sputtered Vanadium films. Structural, surface-morphology and phase-transition properties of the oxidized films as a function of oxidation duration are presented. Phase-pure VO2 films are obtained by oxidizing ~130 nm Vanadium films in short oxidation duration of ~30 seconds. Compared to previous reports on VO2 synthesis using atmospheric oxidation of Vanadium films of similar thickness, we obtain a reduction in oxidation duration by more than one order. Synthesized VO2 thin film shows resistance switching of ~3 orders of magnitude. We demonstrate optical reflectance switching in long-wave infrared wavelengths in VO2 films synthesized using atmospheric oxidation of Vanadium. The extracted refractive index of VO2 in the insulating and in the metallic phase is in good agreement with VO2 synthesized using other methods. The considerable reduction in oxidation time of VO2 synthesis while retaining good resistance and optical switching properties will help in integration of VO2 in limited thermal budget processes, enabling further applications of this phase-transition material.",2105.10264v1 2023-08-18,Magnetoresistance anomaly during the electrical triggering of a metal-insulator transition,"Phase separation naturally occurs in a variety of magnetic materials and it often has a major impact on both electric and magnetotransport properties. In resistive switching systems, phase separation can be created on demand by inducing local switching, which provides an opportunity to tune the electronic and magnetic state of the device by applying voltage. Here we explore the magnetotransport properties in the ferromagnetic oxide (La,Sr)MnO3 (LSMO) during the electrical triggering of an intrinsic metal-insulator transition (MIT) that produces volatile resistive switching. This switching occurs in a characteristic spatial pattern, i.e., the formation of an insulating barrier perpendicular to the current flow, enabling an electrically actuated ferromagnetic-paramagnetic-ferromagnetic phase separation. At the threshold voltage of the MIT triggering, both anisotropic and colossal magnetoresistances exhibit anomalies including a large increase in magnitude and a sign flip. Computational analysis revealed that these anomalies originate from the coupling between the switching-induced phase separation state and the intrinsic magnetoresistance of LSMO. This work demonstrates that driving the MIT material into an out-of-equilibrium resistive switching state provides the means to electrically control of the magnetotransport phenomena.",2308.09260v2 2024-01-30,Picosecond transfer from short-term to long-term memory in analog antiferromagnetic memory device,"Experiments in materials with a compensated ordering of magnetic moments have demonstrated a potential for approaching the thermodynamic limit of the fastest and least-dissipative operation of a digital memory bit. In addition, these materials are very promising for a construction of energy-efficient analog devices with neuromorphic functionalities, which are inspired by computing-in-memory capabilities of the human brain. In this paper, we report on experimental separation of switching-related and heat-related resistance signal dynamics in memory devices microfabricated from CuMnAs antiferromagnetic metal. We show that the memory variable multilevel resistance can be used as a long-term memory (LTM), lasting up to minutes at room temperature. In addition, ultrafast reflectivity change and heat dissipation from nanoscale-thickness CuMnAs films, taking place on picosecond to hundreds of nanoseconds time scales, can be used as a short-term memory (STM). Information about input stimuli, represented by femtosecond laser pulses, can be transferred from STM to LTM after rehearsals at picosecond to nanosecond times in these memory devices, where information can be retrieved at times up to 10^15 longer than the input pulse duration. Our results open a route towards ultra-fast low-power implementations of spiking neuron and synapse functionalities using a resistive analog antiferromagnetic memory.",2401.17370v1 2021-04-21,Machine-Learning Assisted Optimization Strategies for Phase Change Materials Embedded within Electronic Packages,"Leveraging the latent heat of phase change materials (PCMs) can reduce the peak temperatures and transient variations in temperature in electronic devices. But as the power levels increase, the thermal conduction pathway from the heat source to the heat sink limits the effectiveness of these systems. In this work, we evaluate embedding the PCM within the silicon device layer of an electronic device to minimize the thermal resistance between the source and the PCM to minimize this thermal resistance and enhance the thermal performance of the device. The geometry and material properties of the embedded PCM regions are optimized using a combination of parametric and machine learning algorithms. For a fixed geometry, considering commercially available materials, Solder 174 significantly outperforms other organic and metallic PCMs. Also with a fixed geometry, the optimal melting points to minimize the peak temperature is higher than the optimal melting point to minimize the amplitude of the transient temperature oscillation, and both optima increase with increasing heater power. Extending beyond conventional optimization strategies, genetic algorithms and particle swarm optimization with and without neural network surrogate models are used to enable optimization of many geometric and material properties. For the test case evaluated, the optimized geometries and properties are similar between all ML-assisted algorithms, but the computational time depends on the technique. Ultimately, the optimized design with embedded phase change materials reduces the maximum temperature rise by 19% and the fluctuations by up to 88% compared to devices without PCM.",2104.14433v1 2023-10-26,A Critical Assessment of Electronic Structure Descriptors for Predicting Perovskite Catalytic Properties,"The discovery and design of new materials which can efficiently catalyze the oxygen reduction and evolution reactions at reduced temperatures is important for facilitating the widespread adoption of fuel cell and electrolyzer technologies. Numerous studies have produced correlations between catalytic properties, such as oxygen surface exchange or electrode area specific resistance (ASR), and properties of the catalyst material. However, correlations have historically been limited in scope (e.g., using only a few materials or at a single temperature) and it has been difficult to provide detailed assessments of their robustness. Here, we assess the ability of the O p-band center electronic structure descriptor, obtained from density functional theory (DFT) calculations, to correlate with oxygen surface exchange rates, diffusivities, and area specific resistances for a large database of perovskite oxide catalytic properties. By data mining the literature, we obtain 747 catalytic property value data points spanning 299 unique perovskite compositions from 313 studies. We assess linear correlations of each property with the O p-band center and find generally modest correlations that are qualitatively useful (prediction mean absolute errors of about 0.5 log units are typical), where the correlations are improved at higher temperatures (e.g., 800 {\deg}C vs. 500 {\deg}C) and significantly improve when considering fits to the subset of materials which have multiple independent measurements. These findings suggest that the spread of property data is significantly influenced by experimental uncertainty, and subsequent measurements of additional materials will likely improve the O p-band center correlations.",2310.17744v1 1998-11-11,Superconducting Material Diagnostics using a Scanning Near-Field Microwave Microscope,"We have developed scanning near-field microwave microscopes which can image electrodynamic properties of superconducting materials on length scales down to about 2 $\mu$m. The microscopes are capable of quantitative imaging of sheet resistance of thin films, and surface topography. We demonstrate the utility of the microscopes through images of the sheet resistance of a YBa2Cu3O7-d thin film wafer, images of bulk Nb surfaces, and spatially resolved measurements of Tc of a YBa2Cu3O7-d thin film. We also discuss some of the limitations of the microscope and conclude with a summary of its present capabilities.",9811158v1 2001-08-21,Infrared and optical properties of pure and cobalt-doped LuNi_2B_2C,"We present optical conductivity data for Lu(Ni$_{1-x}$Co$_x$)$_2$B$_2$C over a wide range of frequencies and temperatures for x=0 and x=0.09. Both materials show evidence of being good Drude metals with the infrared data in reasonable agreement with dc resistivity measurements at low frequencies. An absorption threshold is seen at approximately 700 cm-1. In the cobalt-doped material we see a superconducting gap in the conductivity spectrum with an absorption onset at 24 +/- 2 cm-1 = 3.9$ +/- 0.4 k_BT_c suggestive of weak to moderately strong coupling. The pure material is in the clean limit and no gap can be seen. We discuss the data in terms of the electron-phonon interaction and find that it can be fit below 600 cm-1 with a plasma frequency of 3.3 eV and an electron-phonon coupling constant lambda_{tr}=0.33 using an alpha^{2}F(omega) spectrum fit to the resistivity.",0108333v1 2005-04-22,Low field magneto-transport in La_0.7Ca_0.3MnO_3-PMMA composites synthesized by polymeric precursor route,"A detailed investigation of the effect of PMMA on the structure, microstructure and magneto-transport properties of manganite La_0.7Ca_0.3MnO_3 (LCMO) is presented. LCMO-PMMA nanostructured composites have been synthesized by a unique polymeric sol-gel route, which leads to improved solubility of PMMA in the LCMO matrix. The LCMO phase is grown in the presence of varying PMMA concentration at ~500 ^0 C. This route yields single phase material and the grain size is observed to decrease slightly with increasing PMMA concentration. On increasing the PMMA concentration, T_C undergoes a small decrease, resistivity is observed to increase by two orders of magnitude, with a concomitant large decrease in T_IM, e.g., from 218 K for virgin LCMO to 108 K for 50 wt% PMMA admixed LCMO. Low field magneto-resistance measured in the temperature range 77-300 K shows considerable enhancement as a function of the PMMA concentration. These phenomena are explained by taking into account the increased intergranular disorder as a consequence of PMMA admixture.",0504579v1 2007-03-01,Magnetic effects at the interface between nonmagnetic oxides,"The electronic reconstruction at the interface between two insulating oxides can give rise to a highly-conductive interface. In analogy to this remarkable interface-induced conductivity we show how, additionally, magnetism can be induced at the interface between the otherwise nonmagnetic insulating perovskites SrTiO3 and LaAlO3. A large negative magnetoresistance of the interface is found, together with a logarithmic temperature dependence of the sheet resistance. At low temperatures, the sheet resistance reveals magnetic hysteresis. Magnetic ordering is a key issue in solid-state science and its underlying mechanisms are still the subject of intense research. In particular, the interplay between localized magnetic moments and the spin of itinerant conduction electrons in a solid gives rise to intriguing many-body effects such as Ruderman-Kittel-Kasuya-Yosida (RKKY) interactions, the Kondo effect, and carrier-induced ferromagnetism in diluted magnetic semiconductors. The conducting oxide interface now provides a versatile system to induce and manipulate magnetic moments in otherwise nonmagnetic materials.",0703028v2 2008-07-09,"Molecular Beam Epitaxy grown (Ga,Mn)(As,P) with perpendicular to plane magnetic easy axis","We present an experimental investigation of the magnetic, electrical and structural properties of Ga0.94Mn0.06As1-yPy layers grown by molecular beam epitaxy on GaAs substrates for y less than or equal to 0.3. X-ray diffraction measurements reveal that the layers are under tensile strain which gives rise to a magnetic easy axis perpendicular to the plane of the layers. The strength of the magnetic anisotropy and the coercive field increase as the phosphorous concentration is increased. The resistivity of all samples shows metallic behaviour with the resistivity increasing as y increases. These materials will be useful for studies of micromagnetic phenomena requiring metallic ferromagnetic material with perpendicular magnetic anisotropy.",0807.1469v1 2009-09-10,"Electric Pulse Induced Resistive Switching, Electronic Phase Separation, and Possible Superconductivity in a Mott insulator","Metal-insulator transitions (MIT) belong to a class of fascinating physical phenomena, which includes superconductivity, and colossal magnetoresistance (CMR), that are associated with drastic modifications of electrical resistance. In transition metal compounds, MIT are often related to the presence of strong electronic correlations that drive the system into a Mott insulator state. In these systems the MIT is usually tuned by electron doping or by applying an external pressure. However, it was noted recently that a Mott insulator should also be sensitive to other external perturbations such as an electric field. We report here the first experimental evidence of a non-volatile electric-pulse-induced insulator-to-metal transition and possible superconductivity in the Mott insulator GaTa4Se8. Our Scanning Tunneling Microscopy experiments show that this unconventional response of the system to short electric pulses arises from a nanometer scale Electronic Phase Separation (EPS) generated in the bulk material.",0909.1978v1 2010-03-13,Ferromagnetic Clusters in the Brownmillerite Bilayered Compounds Ca2.5-xLaxSr0.5GaMn2O8: An Approach to Achieve Layered Spintronics Materials,"We report the effect of La-substitution on the magnetic and magnetotransport properties of Brownmillerite-like bilayered compounds Ca2.5-xLaxSr0.5GaMn2O8 (x = 0, 0.05, 0.075, and 0.1) by using dc-magnetization, resistivity and magnetoresistance techniques. The Rietveld analysis of the room temperature x-ray diffraction patterns confirms no observable change of average crystal structure with the La-substitution. Both magnetic and magnetotransport properties are found to be very sensitive to the La-substitution. Interestingly, the La-substituted compounds show ferromagnetic-like behavior (due to the occurrence of a double exchange mechanism) whereas, the parent compound is an antiferromagnet (TN 150 K). All compounds show an insulating behavior, in the measured temperature range of 100 - 300 K, with an overall decrease in the resistivity with the substitution. A higher value of magnetoresistance has been successfully achieved by the La-substitution. We have proposed an electronic phase separation model, considering the formation of ferromagnetic clusters in the antiferromagnetic matrix, to interpret the observed magnetization and magnetotransport results for the La-substituted samples. The present study demonstrates an approach to achieve new functional materials, based on naturally occurring layered system like Ca2.5-xLaxSr0.5GaMn2O8, for possible spintronics applications.",1003.2685v1 2013-07-24,Large resistivity change and phase transition in LiMnAs,"Antiferromagnetic semiconductors are new alternative materials for spintronic applications and spin valves. In this work, we report a detailed investigation of two antiferromagnetic semiconductors AMnAs (A = Li, LaO), which are isostructural to the well-known LiFeAs and LaOFeAs superconductors. Here we present a comparison between the structural, magnetic, and electronic properties of LiMnAs, LaOMnAs and related materials. Interestingly, both LiMnAs and LaOMnAs show a variation in resistivity with more than five orders of magnitude, making them particularly suitable for use in future electronic devices. From neutron and X-ray diffraction measurements on LiMnAs we have observed a magnetic phase transition corresponding to the Neel temperature of 373.8 K, and a structural transition from the tetragonal to the cubic phase at 768 K. These experimental results are supported by density functional theory (DFT) calculations.",1307.6404v4 2014-03-31,Investigation of Complex Impedance and Modulus Properties of Nd Doped 0.5BiFeO3-0.5PbTiO3 Multiferroic Composites,"0.5BiNdxFe1-xO3-0.5PbTiO3 (x=0.05, 0.10, 0.15, 0.20) composites were successfully synthesized by a solid state reaction technique. At room temperature X-ray diffraction shows tetragonal structure for all concentrations of Nd doped 0.5BiFeO3-0.5PbTiO3 composites. The nature of Nyquist plot confirms the presence of bulk effects only for all compositions of Nd-doped 0.5BiFeO3-0.5PbTiO3 composites. The bulk resistance is found to decreases with the increasing in temperature as well as Nd concentration and exhibits a typical negative temperature coefficient of resistance (NTCR) behavior. Both the complex impedance and modulus studies have suggested the presence of non-Debye type of relaxation in the materials. Conductivity spectra reveal the presence of hopping mechanism in the electrical transport process of the materials. The activation energy of the composite increases with increasing Nd concentration and were found to be 0.28, 0.27, 0.31 and 0.32eV for x=0.05, 0.10, 0.15, 0.20 respectively at 200-275 oC for conduction process.",1403.7981v1 2014-04-09,A new first-principles calculation of field-dependent RF surface impedance of BCS superconductor and application to SRF cavities,"There is a need to better understand the intrinsic limit of radiofrequency (RF) surface impedance that determines the performance of superconducting RF cavities in particle accelerators. Here we present a field-dependent derivation of Mattis-Bardeen (M-B) theory of the RF surface impedance of BCS superconductors based on the shifted Density of States (DoS) resulting from coherently moving Cooper pairs [1].The surprising reduction in resistance with increasing field is explained to be an intrinsic effect. Using this analysis coded in MathematicaTM, survey calculations have been completed which examine the sensitivities of this surface impedance to variation of the BCS material parameters and temperature.Our theoretical prediction of the effective BCS RF surface resistance (Rs) of niobium as a function of peak surface magnetic field amplitude agrees well with recently reported record low loss resonant cavity measurements from Jefferson Lab (JLab) and Fermi National Accelerator Lab (FNAL) with carefully, yet differently, prepared niobium material. The results present a refined description of the ""best theoretical"" performance available to potential applications with corresponding materials. [1]Xiao, B.P., C.E. Reece, and M.J. Kelley, Superconducting surface impedance under radiofrequency field. Physica C: Superconductivity, 2013. 490(0): p. 26-31.",1404.2523v1 2014-11-25,Computing with spins and magnets,"The possible use of spin and magnets in place of charge and capacitors to store and process information is well known. Magnetic tunnel junctions are being widely investigated and developed for magnetic random access memories. These are two terminal devices that change their resistance based on switchable magnetization of magnetic materials. They utilize the interaction between electron spin and magnets to read information from the magnets and write onto them. Such advances in memory devices could also translate into a new class of logic devices that offer the advantage of nonvolatile and reconfigurable information processing over transistors. Logic devices having a transistor-like gain and directionality could be used to build integrated circuits without the need for transistor-based amplifiers and clocks at every stage. We review device characteristics and basic logic gates that compute with spins and magnets from the mesoscopic to the atomic scale, as well as materials, integration, and fabrication challenges and methods.",1411.6960v1 2015-05-22,Direct Method for Calculating Temperature-Dependent Transport Properties,"We show how temperature-induced disorder can be combined in a direct way with first-principles scattering theory to study diffusive transport in real materials. Excellent (good) agreement with experiment is found for the resistivity of Cu, Pd, Pt (and Fe) when lattice (and spin) disorder are calculated from first principles. For Fe, the agreement with experiment is limited by how well the magnetization (of itinerant ferromagnets) can be calculated as a function of temperature. By introducing a simple Debye-like model of spin disorder parameterized to reproduce the experimental magnetization, the temperature dependence of the average resistivity, the anisotropic magnetoresistance and the spin polarization of a Ni$_{80}$Fe$_{20}$ alloy are calculated and found to be in good agreement with existing data. Extension of the method to complex, inhomogeneous materials as well as to the calculation of other finite-temperature physical properties within the adiabatic approximation is straightforward.",1505.06231v1 2015-11-04,Numerical Calculations of Wake Fields and Impedances of LHC Collimators' Real Structures,"The LHC collimators have very complicated mechanical designs including movable jaws made of higly resistive materials, ferrite materials, tiny RF contacts. Since the jaws are moved very close to the circulating beams their contribution in the overall LHC coupling impedance is dominant, with respect to other machine components. For these reasons accurate simulation of collimators' impedance becomes very important and challenging. Besides, several dedicated tests have been performed to verify correct simulations of lossy dispersive material properties, such as resistive wall and ferrites, benchmarking code results with analytical, semi-analytical and other numerical codes outcomes. Here we describe all the performed numerical tests and discuss the results of LHC collimators' impedances and wake fields calculations.",1511.01236v1 2016-04-19,Metallicity and conductivity crossover in white light illuminated CH$_3$NH$_3$PbI$_3$ perovskite,"The intrinsic d.c. electrical resistivity ($\rho$) - measurable on single crystals only - is often the quantity first revealing the properties of a given material. In the case of CH$_3$NH$_3$PbI$_3$ perovskite measuring $\rho$ under white light illumination provides insight into the coexistence of extended and shallow localized states (0.1 eV below the conduction band). The former ones dominate the electrical conduction while the latter, coming from neutral defects, serve as a long-lifetime charge carrier reservoir accessible for charge transport by thermal excitation. Remarkably, in the best crystals the electrical resistivity shows a metallic behaviour under illumination up to room temperature, giving a new dimension to the material in basic physical studies.",1604.05637v1 2016-05-13,Quantifying structure-property relationships during resistance spot welding of an aluminum 6061-T6 joint,"Microstructure-property relationships of resistance spot welded 6061-T6 aluminum alloy lap joints were investigated via mechanical testing and microscopy techniques. Quasi-static tensile and novel shear punch tests were employed to measure the mechanical properties of the distinct weld regions. Quasi-static tensile and shear punch tests revealed constantly decreasing strength and ductility as the weld center was approached. For instance, the ultimate tensile strength of the fusion zone decreased by ~52% from the parent material (341 MPa to 162 MPa) while the yield strength decreased by ~62% (312 MPa to 120 MPa). The process-induced microstructures were analyzed with scanning electron microscopy and optical microscopy to elucidate the underlying cause of the reduced mechanical properties. Fractography reveals void growth from particles being the dominant damage mechanism in the parent material as compared to void nucleation in the fusion zone. Overall, significant changes in the mechanical behavior across the weld are the result of a change in microstructure congruent with a loss of T6 condition (precipitate coarsening).",1605.04251v1 2016-06-17,Electronic ground state of MnB$_{4}$,"Recent studies have dealt with the electronic and magnetic ground state properties of the tetraboride material MnB$_4$. So far, however, the ground state properties could not be established unambiguously. Therefore, here we present an experimental study on single-crystalline MnB$_4$ by means of resistivity and magnetization measurements. For this, we have developed a sample holder that allows four-point ac resistivity measurements on these very small ($\sim$\,100\,$\mu$m) samples. With our data we establish that the electronic ground state of MnB$_4$ is intrinsically that of a pseudo-gap system, in agreement with recent band structure calculations. Furthermore, we demonstrate that the material does neither show magnetic order nor a behavior arising from the vicinity to a magnetically ordered state, this way disproving previous claims.",1606.05484v3 2016-12-15,Superconductivity above 500 K in conductors made by bringing n-alkane into contact with graphite,"In 1986, a cuprate superconductor (Ba-La-Cu-O system) having a critical temperature which goes over the BCS limit (~30 K) was discovered and then a cuprate superconductor (Y-Ba-Cu-O system) with a critical temperature higher than 77 K was discovered. Furthermore, a Hg-based cuprate with a critical temperature of 133 K was found. The 133 K is still the highest critical temperature of conventional superconductors under atmospheric pressure. We have shown that materials obtained by bringing n-alkanes into contact with graphite are capable of conducting electricity with almost no energy loss at room temperature. We here report that the sudden jump in resistance showing a phase transition is observed in the materials during heating by two-probe resistance measurement. The measured critical temperatures of the materials consisting of pitch-based graphite fibers and n-alkanes having 7-16 carbon atoms range from 363.08 to 504.24 K and the transition widths range between 0.15 and 3.01 K. We also demonstrate that superconductors with critical temperatures beyond 504 K are obtained by alkanes with 16 or more carbon atoms.",1612.05294v1 2017-02-20,Gate Tunable Magneto-resistance of Ultra-Thin WTe2 Devices,"In this work, the magneto-resistance (MR) of ultra-thin WTe2/BN heterostructures far away from electron-hole equilibrium is measured. The change of MR of such devices is found to be determined largely by a single tunable parameter, i.e. the amount of imbalance between electrons and holes. We also found that the magnetoresistive behavior of ultra-thin WTe2 devices is well-captured by a two-fluid model. According to the model, the change of MR could be as large as 400,000%, the largest potential change of MR among all materials known, if the ultra-thin samples are tuned to neutrality when preserving the mobility of 167,000 cm2V-1s-1 observed in bulk samples. Our findings show the prospects of ultra-thin WTe2 as a variable magnetoresistance material in future applications such as magnetic field sensors, information storage and extraction devices, and galvanic isolators. The results also provide important insight into the electronic structure and the origin of the large MR in ultra-thin WTe2 samples.",1702.05876v1 2017-10-05,Multi-scale Modeling of Plasticity Nearby Precipitates in Nanostructured Materials,"Precipitation strengthening is one of the most effective methods to design alloys with the desired combination of strength and ductility. The main mechanism of strengthening is generally known to be the interaction between dislocations and precipitates. When a dislocation encounters a precipitate, it bends and therefore the level of applied stress to the precipitate increases. Once the applied stress reaches the precipitate resistance, it passes the precipitate. Dislocations can bypass precipitates either by forming the Orowan loops or by cutting them. In this research, the focus is set on a small domain nearby precipitates to investigate their effects on the effective plastic strain. Both penetrable and impenetrable precipitates are considered. Two scales are coupled to model this phenomenon, the nano-micro scale where plasticity is determined by explicit three-dimensional discrete dislocation dynamics analysis and the continuum scale where the finite element method is applied. With this hybrid approach, complex problems in plastic deformation of nanostructured materials can be addressed. Finally, the relation between the precipitate resistance and the effective plastic strain is investigated.",1710.02075v3 2018-05-03,Enhanced Electron Transport in Thin Copper Films via Atomic-Layer Materials Capping,"Using first-principles calculations based on density functional theory and non-equilibrium Green's functions, we characterized the effect of surface termination on the electronic transport properties of nanoscale Cu slabs. With ideal, clean (111) surfaces and oxidized ones as baselines we explore the effect of capping the slabs with graphene, hexagonal boron nitrate, molybdenum disulfide and stanene. Surface oxide suppresses balistic conductance by a factor of 10 compared to the ideal surface. Capping the ideal copper surface with graphene slightly increase conductance but MoS$_2$ and stanene have the opposite effect due to stronger interactions at the interface. Interestingly, we find that capping atomistically roughed copper surfaces with graphene or MoS$_2$ decreases the resistance per unit length by 20 and 13%, respectively, due to reduced scattering. The results presented in this work suggest that two-dimensional materials can be used as an ultra-thin liner in metallic interconnect technology without increasing the interconnect line resistivity significantly.",1805.01517v1 2018-06-07,On the magnetic and electronic properties of NpPdSn,"We have studied NpPdSn by means of the heat capacity, electrical resistivity, Seebeck and Hall effect, $^{237}$Np M\""{o}ssbauer spectroscopy, and neutron diffraction measurements in the temperature range 2-300 K and under magnetic fields up to 14 T. NpPdSn orders antiferromagnetically below the N\'eel temperature $T_N$ = 19 K and shows localized magnetism of Np$^{3+}$ ion with a a doubly degenerate ground state. In the magnetic state the electrical resistivity and heat capacity are characterized by electron-magnon scattering with spin-waves spectrum typical of anisotropic antiferromagnets. An enhanced Sommerfeld coefficient and typical behavior of magnetorestistivity, Seebeck and Hall coefficients are all characteristic of systems with strong electronic correlations. The low temperature antiferromagnetic state of NpPdSn is verified by neutron diffraction and $^{237}$Np M\""{o}ssbauer spectroscopy and possible magnetic structures are discussed.",1806.02879v1 2019-09-06,Unveiling multiferroic proximity effect in graphene,"We demonstrate that electronic and magnetic properties of graphene can be tuned via proximity of multiferroic substrate. Our first-principles calculations performed both with and without spin-orbit coupling clearly show that by contacting graphene with bismuth ferrite BiFeO$_3$ (BFO) film, the spin-dependent electronic structure of graphene is strongly impacted both by the magnetic order and by electric polarization in the underlying BFO. Based on extracted Hamiltonian parameters obtained from the graphene band structure, we propose a concept of six-resistance device based on exploring multiferroic proximity effect giving rise to significant proximity electro- (PER), magneto- (PMR), and multiferroic (PMER) resistance effects. This finding paves a way towards multiferroic control of magnetic properties in two dimensional materials.",1909.02844v1 2017-01-27,Strain-modulated Bandgap and Piezo-resistive Effect in Black Phosphorus Field-effect Transistors,"Energy bandgap largely determines the optical and electronic properties of a semiconductor. Variable bandgap therefore makes versatile functionality possible in a single material. In layered material black phosphorus, the bandgap can be modulated by the number of layers; as a result, few-layer black phosphorus has discrete bandgap values that are relevant for opto-electronic applications in the spectral range from red, in monolayer, to mid-infrared in the bulk limit. Here, we further demonstrate continuous bandgap modulation by mechanical strain applied through flexible substrates. The strain-modulated bandgap significantly alters the charge transport in black phosphorus at room temperature; we for the first time observe a large piezo-resistive effect in black phosphorus field-effect transistors (FETs). The effect opens up opportunities for future development of electro-mechanical transducers based on black phosphorus, and we demonstrate strain gauges constructed from black phosphorus thin crystals.",1701.08041v1 2019-07-27,Microwave derived monoclinic Ba1-xSnxNb2O6 materials as an alternative of ITO,"Microwave synthesis was optimized for preparing novel monoclinic Tin-doped Barium Niobate ceramics (Ba1-xSnxNb2O6; x= 0.0, 0.01, 0.05, 0.1, 0.2, 0.3) BSN. The intensity of monoclinic phase formation was observed to decrease on increasing tin as dopant indicating decreased crystallinity. Strained crystalline phase was observed in undoped sample that became severe on doping tin. Monoclinic metal alloy Sn2O3 formation was confirmed on increasing tin doping beyond 5%. Electronic configuration of tin (II) oxide supports the local site-wise monoclinic disorder in crystal structure due to sterically active lone pair. Such a disorder arranges increased number of degenerate energy states and reduce effective energy gap between conduction band minimum and valence band maximum. All BSN compositions were investigated for monoclinic phase stabilization, ultra-violet absorption, dielectric response, raman modes and type of carrier concentration along with hall resistivity. All measurements possessed inflexion corresponding to 5 atomic % tin doping indicating successful site substitution and estimated Sn2O3 metal formation beyond this. The values of reducing optical energy band gap, transparency to visible spectrum and hall resistivity indicated utility of these materials as a substitute transparent conducting oxide (TCO) for well-known indium tin oxide (ITO).",1907.11946v1 2019-04-24,Progressive amorphization of GeSbTe phase-change material under electron beam irradiation,"Fast and reversible phase transitions in chalcogenide phase-change materials (PCMs), in particular, Ge-Sb-Te compounds, are not only of fundamental interests, but also make PCMs based random access memory (PRAM) a leading candidate for non-volatile memory and neuromorphic computing devices. To RESET the memory cell, crystalline Ge-Sb-Te has to undergo phase transitions firstly to a liquid state and then to an amorphous state, corresponding to an abrupt change in electrical resistance. In this work, we demonstrate a progressive amorphization process in GeSb2Te4 thin films under electron beam irradiation on transmission electron microscope (TEM). Melting is shown to be completely absent by the in situ TEM experiments. The progressive amorphization process resembles closely the cumulative crystallization process that accompanies a continuous change in electrical resistance. Our work suggests that if displacement forces can be implemented properly, it should be possible to emulate symmetric neuronal dynamics by using PCMs.",1904.10601v2 2015-06-02,Nonmonotonic fracture behavior of polymer nanocomposites,"Polymer composite materials are widely used for their exceptional mechanical properties, notably their ability to resist large deformations. Here we examine the failure stress and strain of rubbers reinforced by varying amounts of nano-sized silica particles. We find that small amounts of silica increase the fracture stress and strain, but too much filler makes the material become brittle and consequently fracture happens at small deformations. We thus find that as a function of the amount of filler there is an optimum in the breaking resistance at intermediate filler concentrations. We use a modified Griffith theory to establish a direct relation between the material properties and the fracture behavior that agrees with the experiment.",1506.00832v1 2015-07-23,Tuning bad metal and non-Fermi liquid behavior in a Mott material: rare earth nickelate thin films,"Resistances that exceed the Mott-Ioffe-Regel limit, known as bad metal behavior, and non-Fermi liquid behavior are ubiquitous features of the normal state of many strongly correlated materials. Here we establish the conditions that lead to bad metal and non-Fermi liquid phases in NdNiO3, which exhibits a prototype, bandwidth-controlled metal-insulator transition. We show that resistance saturation is determined by the magnitude of the Ni eg orbital splitting, which can be tuned by strain in epitaxial films, causing the appearance of bad metal behavior under certain conditions. The results shed light on the nature of a crossover to non-Fermi liquid metal phase and provide a predictive criterion for strong localization. They elucidate a seemingly complex phase behavior as a function of film strain and confinement and provide guidelines for orbital engineering and novel devices.",1507.06619v1 2018-07-17,Current jetting distorted planar Hall effect in a Weyl semimetal with ultrahigh mobility,"A giant planar Hall effect (PHE) and anisotropic magnetoresistance (AMR) is observed in TaP, a nonmagnetic Weyl semimetal with ultrahigh mobility. The perpendicular resistivity (i.e., the planar magnetic field applied normal to the current) far exceeds the zero-field resistivity, which thus rules out the possible origin of negative longitudinal magnetoresistance. The giant PHE/AMR is finally attributed to the large anisotropic orbital magnetoresistance that stems from the ultrahigh mobility. Furthermore, the mobility-enhanced current jetting effects are found to strongly deform the line shape of the curves, and their evolution with the changing magnetic field and temperature is also studied. Although the giant PHE/AMR suggests promising applications in spintronics, the enhanced current jetting shows the other side of the coin, which needs to be considered in the future device design.",1807.06229v3 2019-01-03,Realization of Kondo chain in CeCo$_2$Ga$_8$,"We revisited the anisotropy of the heavy-fermion material CeCo$_2$Ga$_8$ by measuring the electrical resistivity and magnetic susceptibility along all the principal $\mathbf{a}$-, $\mathbf{b}$- and $\mathbf{c}$-axes. Resistivity along $\mathbf{c}$-axis ($\rho_c$) shows clear Kondo coherence below about 17 K, while both $\rho_{a}$ and $\rho_{b}$ remain incoherent down to 2 K. The magnetic anisotropy is well understood within the theoretical frame of crystalline electric field effect in combination with magnetic exchange interactions. We found the anisotropy ratio of these magnetic exchange interactions, $|J_{ex}^c/J_{ex}^{a,b}|$, reaches a large value of 4-5. We, therefore, firmly demonstrate that CeCo$_2$Ga$_8$ is a quasi-one-dimensional heavy-fermion compound both electrically and magnetically, and thus provide a realistic example of \textit{Kondo chain}.",1901.00558v2 2019-01-04,Experimental and Numerical Investigation of the Fracture Behavior of Particle Reinforced Alkali Activated Slag Mortars,"This paper presents fracture response of alkali-activated slag (AAS) mortars with up to 30% (by volume) of slag being replaced by waste iron powder which contains a significant fraction of elongated particles. The elongated iron particles act as micro-reinforcement and improve the crack resistance of AAS mortars by increasing the area of fracture process zone (FPZ). Increased area of FPZ signifies increased energy-dissipation which is reflected in the form of significant increase in the crack growth resistance as determined from R-curves. Fracture response of notched AAS mortar beams under three-point bending is simulated using extended finite element method (XFEM) to develop a tool for direct determination of fracture characteristics such as crack extension and fracture toughness in particulate-reinforced AAS mortars. Fracture response simulated using the XFEM based framework correlates well with experimental observations. The comprehensive fracture studies reported here provide an economical and sustainable means towards improving the ductility of AAS systems which are generally more brittle than their conventional ordinary portland cement counterparts.",1901.01025v1 2019-10-17,The grain-size effect on thermal conductivity of uranium dioxide,"We have investigated the grain boundary scattering effect on the thermal transport behavior of uranium dioxide (UO$_2$). The polycrystalline samples having different grain-sizes (0.125, 1.8, and 7.2 $\mu$m) have been prepared by spark plasma sintering technique and characterized by x-ray powder diffraction (XRD), scanning electron microscope (SEM), and Raman spectroscopy. The thermal transport properties (the thermal conductivity and thermoelectric power) have been measured in the temperature range 2-300~K and the results were analyzed in terms of various physical parameters contributing to the thermal conductivity in these materials in relation to grain-size. We show that thermal conductivity decreases systematically with lowering grain-size in the temperatures below 30 K, where the boundary scattering dominates the thermal transport. At higher temperatures more scattering processes are involved in the heat transport in these materials, making the analysis difficult. We determined the grain boundary Kapitza resistance that would result in the observed increase in thermal conductivity with grain size, and compared the value with Kapitza resistances calculated for UO$_2$ using molecular dynamics from the literature.",1910.08014v1 2020-01-06,Transport characteristics of type II Weyl semimetal MoTe2 thin films grown by chemical vapor deposition,"Theoretical calculations and experimental observations show MoTe2 is a type II Weyl semimetal, along with many members of transition metal dichalcogenides family. We have grown highly crystalline large-area MoTe2 thin films on Si/SiO2 substrates by chemical vapor deposition. Very uniform, continuous, and smooth films were obtained as confirmed by scanning electron microscopy and atomic force microscopy analyses. Measurements of the temperature dependence of longitudinal resistivity and current-voltage characteristics at different temperature are discussed. Unsaturated, positive quadratic magnetoresistance of the as-grown thin films has been observed from 10 K to 200 K. Hall resistivity measurements confirm the majority charge carriers are hole.",2001.01703v1 2020-05-11,Skyrmion phase in MnSi on sapphire grown by a conventional sputtering,"Topologically protected chiral skyrmion is an intriguing spin texture, which has attracted much attention because of fundamental research and future spintronic applications. MnSi with the non-centrosymmetric structure is well-known material hosting skyrmion phase. To date, preparation of MnSi crystals has been investigated by using special instruments with ultrahigh vacuum chamber. Here, we introduce a facile way to grow MnSi films on sapphire, which is in relatively low vacuum environment of conventional magnetron sputtering. Magnetotransport properties including Hall resistivity measurements allow to confirm the existence of skyrmion phase in MnSi film. Because as-grown MnSi films on sapphire has polycrystalline nature, the emergent features of skyrmion phase are limited and complicated. However, we observed the stable skyrmion phase in a broad range of temperatures and magnetic fields, which is explained by phenomenological scaling analyses of Hall resistivities contribution. Our findings provide not only a general way to prepare the materials possessing skyrmion phase, but also insight into further research to stimulate more degrees of freedom in our inquisitiveness.",2005.04841v1 2020-08-11,"Anomalous Hall effect in half-metallic Heusler compound Co$_{2}$Ti$X$ ($X$=Si, Ge)","Though Weyl fermions have recently been observed in several materials with broken inversion symmetry, there are very few examples of such systems with broken time reversal symmetry. Various Co$_{2}$-based half-metallic ferromagnetic Heusler compounds are lately predicted to host Weyl type excitations in their band structure. These magnetic Heusler compounds with broken time reversal symmetry are expected to show a large momentum space Berry curvature, which introduces several exotic magneto-transport properties. In this report, we present systematic analysis of experimental results on anomalous Hall effect (AHE) in Co$_2$Ti$X$ ($X$=Si and Ge). This study is an attempt to understand the role of Berry curvature on AHE in Co$_2$Ti$X$ family of materials. The anomalous Hall resistivity is observed to scale quadratically with the longitudinal resistivity for both the compounds. The detailed analysis indicates that in anomalous Hall conductivity, the intrinsic Karplus-Luttinger Berry phase mechanism dominates over the extrinsic skew scattering and side-jump mechanism.",2008.04837v1 2021-03-24,Manipulating Berry curvature of SrRuO3 thin films via epitaxial strain,"Berry curvature plays a crucial role in exotic electronic states of quantum materials, such as intrinsic anomalous Hall effect. As Berry curvature is highly sensitive to subtle changes of electronic band structures, it can be finely tuned via external stimulus. Here, we demonstrate in SrRuO3 thin films that both the magnitude and sign of anomalous Hall resistivity can be effectively controlled with epitaxial strain. Our first-principles calculations reveal that epitaxial strain induces an additional crystal field splitting and changes the order of Ru d orbital energies, which alters the Berry curvature and leads to the sign and magnitude change of anomalous Hall conductivity. Furthermore, we show that the rotation of Ru magnetic moment in real space of tensile strained sample can result in an exotic nonmonotonic change of anomalous Hall resistivity with the sweeping of magnetic field, resembling the topological Hall effect observed in non-coplanar spin systems. These findings not only deepen our understanding of anomalous Hall effect in SrRuO3 systems, but also provide an effective tuning knob to manipulate Berry curvature and related physical properties in a wide range of quantum materials.",2103.12973v1 2022-06-06,Anomalous Transport Properties of Re$_3$Ge$_7$,"Single crystals of intermetallic Re$_3$Ge$_7$ were grown and characterized by measuring magnetization, electrical resistivity, Hall coefficient, and specific heat. Magnetization measurements show the material is weakly diamagnetic. A phase transition is indicated by a kink in magnetic susceptibility at $T_{c} = 58.5$K and is confirmed by a $\lambda$-like anomaly in specific heat. In zero-field, the temperature dependence of electrical resistivity $\rho(T)$ follows a typical metallic behavior above $T_c$ and sharply increases below $T_c$, showing a metal-to-insulator-like transition. When a magnetic field is applied, strong effects on the transport properties are observed. The temperature dependence of magnetoresistivity $\Delta\rho$ = $\rho (T, H)$ - $\rho (T, H=0)$ develops a maximum around 30 K, deviating from ordinary metallic behavior. Analysis of the Hall coefficient measurements indicates that the carrier density is 0.04 per formula unit at 300 K and drops by two orders of magnitude below $T_c$. The effective mass of charge carriers is inferred from the analysis of the Shubnikov-de Haas quantum oscillations to be close to the bare electron mass.",2206.02943v1 2022-06-28,Colossal piezoresistance in narrow-gap Eu5In2Sb6,"Piezoresistance, the change of a material's electrical resistance ($R$) in response to an applied mechanical stress ($\sigma$), is the driving principle of electromechanical devices such as strain gauges, accelerometers, and cantilever force sensors. Enhanced piezoresistance has been traditionally observed in two classes of uncorrelated materials: nonmagnetic semiconductors and composite structures. We report the discovery of a remarkably large piezoresistance in Eu$_5$In$_2$Sb$_6$ single crystals, wherein anisotropic metallic clusters naturally form within a semiconducting matrix due to electronic interactions. Eu$_5$In$_2$Sb$_6$ shows a highly anisotropic piezoresistance, and uniaxial pressure along [001] of only 0.4~GPa leads to a resistivity drop of more than 99.95\% that results in a colossal piezoresistance factor of $5000\times10^{-11}$Pa$^{-1}$. Our result not only reveals the role of interactions and phase separation in the realization of colossal piezoresistance, but it also highlights a novel route to multi-functional devices with large responses to both pressure and magnetic field.",2206.14073v1 2022-07-06,Sn2Pd: a possible superconducting material with topological surface states,"In this article, we report the detailed magneto transport measurements of the topological semimetal (TSM) candidate, Sn2Pd. Single crystal of Sn2Pd is synthesized through the self-flux method. Phase purity and crystalline morphology are confirmed through powder X ray diffraction (PXRD) pattern and field emission scanning electron microscopy (FESEM) image. Signatures of superconducting transition are seen in both transport and magneto transport measurements, which are further supported by the AC magnetization studies. Sn2Pd is found to show superconductivity onset at below 2.8K, but not the zero resistivity down to 2K. Although, isothermal magneto resistivity measurements below superconducting onset (2.8K) clearly exhibited superconductor-like behavior, but is not observed in heat capacity measurements, indicating the same to be of weak nature. Magnetotransport measurements performed in a normal state of Sn2Pd show the presence of a weak antilocalization (WAL) effect, which is confirmed by modeling of low field magneto-conductivity (MC) through Hikami Larkin Nagaoka (HLN) formalism. Here, it is worth mentioning that the present article is the first report on magneto transport measurements of Sn2Pd, which show the same to be a topological material with a weak superconducting phase below around 2.8K.",2207.02579v1 2023-03-17,On the determination of the thermal shock parameter of MAX phases: A combined experimental-computational study,"Thermal shock resistance is one of the performance-defining properties for applications where extreme temperature gradients are required. The thermal shock resistance of a material can be described by means of the thermal shock parameter RT. Here, the thermo-mechanical properties required for the calculation of RT are quantum-mechanically predicted, experimentally determined, and compared for Ti3AlC2 and Cr2AlC MAX phases. The coatings are synthesized utilizing direct current magnetron sputtering without additional heating, followed by vacuum annealing. It is shown that the RT of both Ti3AlC2 and Cr2AlC obtained via simulations are in good agreement with the experimentally obtained ones. Comparing the MAX phase coatings, both experiments and simulations indicate superior thermal shock behavior of Ti3AlC2 compared to Cr2AlC, attributed primarily to the larger linear coefficient of thermal expansion of Cr2AlC. The results presented herein underline the potential of ab initio calculations for predicting the thermal shock behavior of ionically-covalently bonded materials.",2303.10266v2 2023-05-18,Observation and enhancement of room temperature bilinear magnetoelectric resistance in sputtered topological semimetal Pt3Sn,"Topological semimetal materials have become a research hotspot due to their intrinsic strong spin-orbit coupling which leads to large charge-to-spin conversion efficiency and novel transport behaviors. In this work, we have observed a bilinear magnetoelectric resistance (BMER) of up to 0.1 nm2A-1Oe-1 in a singlelayer of sputtered semimetal Pt3Sn at room temperature. Different from previous observations, the value of BMER in sputtered Pt3Sn does not change out-of-plane due to the polycrystalline nature of Pt3Sn. The observation of BMER provides strong evidence of the existence of spin-momentum locking in the sputtered polycrystalline Pt3Sn. By adding an adjacent CoFeB magnetic layer, the BMER value of this bilayer system is doubled compared to the single Pt3Sn layer. This work broadens the material system in BMER study, which paves the way for the characterization of topological states and applications for spin memory and logic devices.",2305.10720v2 2023-09-12,In operando cryo-STEM of pulse-induced charge density wave switching in TaS$_2$,"The charge density wave (CDW) material 1T-TaS$_2$ exhibits a pulse-induced insulator-to-metal transition, which shows promise for next-generation electronics such as memristive memory and neuromorphic hardware. However, the rational design of TaS$_2$ devices is hindered by a poor understanding of the switching mechanism, the pulse-induced phase, and the influence of material defects. Here, we operate a 2-terminal TaS$_2$ device within a scanning transmission electron microscope (STEM) at cryogenic temperature, and directly visualize the changing CDW structure with nanoscale spatial resolution and down to 300 {\mu}s temporal resolution. We show that the pulse-induced transition is driven by Joule heating, and that the pulse-induced state corresponds to nearly commensurate and incommensurate CDW phases, depending on the applied voltage amplitude. With our in operando cryo-STEM experiments, we directly correlate the CDW structure with the device resistance, and show that dislocations significantly impact device performance. This work resolves fundamental questions of resistive switching in TaS$_2$ devices critical for engineering reliable and scalable TaS$_2$ electronics.",2309.06406v1 2024-05-15,Laser Printing of Silver and Silver Oxide,"We show that direct laser writing (DLW) in aqueous silver nitrate with a 1030 nm femtosecond (fs) laser results in deposition of a mixture of silver oxide and silver, in contrast to the pure silver deposition previously reported with 780 nm fs DLW. However, adding photoinitiator prevents silver oxide formation in a concentration-dependent manner. As a result, the resistivity of the material can also be controlled by photoinitiator concentration with resistivity being reduced from approximately 9e-3 $\Omega m$ to 3e-7 $\Omega m$. Silver oxide peaks dominate the X-ray diffraction spectra when no photoinitiator is present, while the peaks disappear with photoinitiator concentrations above 0.05wt%. While femtosecond pulses are needed to initiate deposition, a continues-wave laser when well overlapped with the previously written material and supplying enough average power can lead to further printing, suggesting thermal deposition can also occur where the photoinitiator molecule also acts as a general reducing agent that prevents oxide formation. We also compare the surface quality of printed lines for different photoinitiator concentrations and laser printing conditions. A THz polarizer and metamaterial are printed as a demonstration of silver oxide printing.",2405.09340v1 2022-03-15,High Rate and High Precision Timing and Calorimeter Detectors,"High precision timing, high rate calorimeters, and radiation resistance are becoming an important issue in particle physics especially in Energy and Intensity Frontiers. We discuss doped Zinc Oxide (ZnO:Ga or GZO; ZnO:X where X is Al, Cu or others) as a very fast scintillator and wavelength shifter (WLS), Total internal reflection films, and PMT capable of counting at 300 MHz with 10 ps timing precision, with superior radiation resistance.",2203.09942v1 1998-01-20,"QHE, magnetoresistance and disordered transport on 2D mesoscopic plaquettes","The transport properties of a rectangular mesoscopic plaquette in the presence of a perpendicular magnetic field are studied in a tight-binding model with randomly distributed traps. The longitudinal and Hall resistances are calculted in the four-probe Landauer-B\""{u}ttiker formalism which accounts automatically both for the quantum coherence and the trapping-induced localization. The localized character of eigenvectors and the specific aspect of the density of states at a given magnetic flux are correlated with the behaviour of the mentioned resistances as function of the Fermi energy. The Hall insulator and quantum Hall regimes are evidentiated. The dependence on magnetic field of the configurational averages of the longitudinal and Halll resistance is studied in a purely quantum-mechanical approach. Both negative and positive magnetoresistances are found.",9801192v1 1998-07-16,Low temperature resistivity in a nearly half-metallic ferromagnet,"We consider electron transport in a nearly half-metallic ferromagnet, in which the minority spin electrons close to the band edge at the Fermi energy are Anderson-localized due to disorder. For the case of spin-flip scattering of the conduction electrons due to the absorption and emission of magnons, the Boltzmann equation is exactly soluble to the linear order. From this solution we calculate the temperature dependence of the resistivity due to single magnon processes at sufficiently low temperature, namely $k_BT\ll D/L^2$, where $L$ is the Anderson localization length and $D$ is the magnon stiffness. And depending on the details of the minority spin density of states at the Fermi level, we find a $T^{1.5}$ or $T^{2}$ scaling behavior for resistivity. Relevance to the doped perovskite manganite systems is discussed.",9807244v1 1998-11-26,Kinetics of electric field induced oxygen ion migration in epitaxial metallic oxide films,"In this paper we report the observation of curent induced change of resistance of thin metallic oxide films. The resistance changes at a very low current (current density $J \geq 10^{3}$ A/cm$^{2}$). We find that the time dependence associated with the processes (increase of resistance) show a streched exponential type dependence at lower temperature, which crosses over to a creep type behavior at $T \geq$ 350 K. The time scale associated shows a drastic drop in the magnitude at $T \approx$ 350 K, where a long range diffusion sets in increasing the conductivity noise. The phenomena is like a ""glass-transition"" in the random lattice of oxygen ions.",9811377v1 1999-09-14,Anomalous temperature behavior of resistivity in lightly doped manganites around a metal-insulator phase transition,"An unusual temperature and concentration behavior of resistivity in $La_{0.7}Ca_{0.3}Mn_{1-x}Cu_xO_3$ has been observed at slight $Cu$ doping ($0\leq x \leq 0.05$). Namely, introduction of copper results in a splitting of the resistivity maximum around a metal-insulator transition temperature $T_0(x)$ into two differently evolving peaks. Unlike the original $Cu$-free maximum which steadily increases with doping, the second (satellite) peak remains virtually unchanged for $x 20 kOe) is observed in a much broader temperature range. This effect is not only frequency- dependent, but also highly sensitive to anisotropy. We call it anisotropic AC magnetoresistance.",9912259v2 2000-07-31,Electrical transport properties of bulk Ni$_{c}$Fe$_{1-c}$ alloys and related spin-valve systems,"Within the Kubo-Greenwood formalism we use the fully relativistic, spin-polarized, screened Korringa-Kohn-Rostoker method together with the coherent-potential approximation for layered systems to calculate the resistivity for the permalloy series Ni$_{c}$Fe$_{1-c}$. We are able to reproduce the variation of the resistivity across the entire series; notably the discontinuous behavior in the vicinity of the structural phase transition from bcc to fcc. The absolute values for the resistivity are within a factor of two of the experimental data. Also the giant magnetoresistance of a series of permalloy-based spin-valve structures is estimated; we are able to reproduce the trends and values observed on prototypical spin-valve structures.",0007507v1 2001-10-19,"Transport, magnetic, thermodynamic and optical properties in Ti-doped Sr_2RuO_4","We report on electrical resistivity, magnetic susceptibility and magnetization, on heat capacity and optical experiments in single crystals of Sr_2Ru_(1-x)Ti_xO_4. Samples with x=0.1 and 0.2 reveal purely semiconducting resistivity behavior along c and the charge transport is close to localization within the ab-plane. A strong anisotropy in the magnetic susceptibility appears at temperatures below 100 K. Moreover magnetic ordering in c-direction with a moment of order 0.01 mu_B/f.u. occurs at low temperatures. On doping the low-temperature linear term of the heat capacity becomes reduced significantly and probably is dominated by spin fluctuations. Finally, the optical conductivity reveals the anisotropic character of the dc resistance, with the in-plane conductance roughly following a Drude-type behavior and an insulating response along c.",0110412v1 2002-01-10,Linear and nonlinear regime of a Random Resistor Network under biased percolation,"We investigate the steady state of a two-dimensional random resistor network subjected to two competing biased percolations as a function of the bias strength. The properties of the linear and nonlinear regimes are studied by means of Monte Carlo simulations. In constant current conditions, a scaling relation is found between $/_0$ and $I/I_0$, where $$ is the average network resistance, $_0$ the Ohmic resistance and $I_0$ an appropriate threshold value for the onset of nonlinearity. A similar scaling relation is found also for the relative variance of resistance fluctuations. These results are in good agreement with electrical breakdown measurements performed in composite materials.",0201152v1 2002-04-11,In-plane Anisotropy on Resistivity and Thermopower in The Misfit Layered Oxide Bi2-xPbxSr2Co2Oy,"We investigated the in-plane anisotropy on the resistivity and thermopower of Bi2-xPbxSr2Co2Oy single crystals, which have a misfit structure between the hexagonal CoO2 layer and the rock salt Bi2Sr2O4 layer. The resistivity and thermopower show significantly large anisotropy, which exceeds two at maximum. This anisotropy would come from the anisotropic pseudogap formation enhanced by the misfit structure. The thermopower changes with Pb doping to take a maximum at x=0.4. The misfit structure improves the thermoelectric properties through chemical pressure. The power factor is as large as 9 muW/cmK2 at 100 K for x=0.6, which is the highest value for thermoelectric oxides at 100 K.",0204245v1 2002-05-23,Nonlinear AC resistivity in s-wave and d-wave disordered granular superconductors,"We model s-wave and d-wave disordered granular superconductors with a three-dimensional lattice of randomly distributed Josephson junctions with finite self-inductance. The nonlinear ac resistivity of these systems was calculated using Langevin dynamical equations. The current amplitude dependence of the nonlinear resistivity at the peak position is found to be a power law characterized by exponent $\alpha$. The later is not universal but depends on the self-inductance and current regimes. In the weak current regime $\alpha$ is independent of the self-inductance and equal to 0.5 or both of s- and d-wave materials. In the strong current regime this exponent depends on the screening. We find $\alpha \approx 1$ for some interval of inductance which agrees with the experimental finding for d-wave ceramic superconductors.",0205475v1 2002-12-06,Ab initio and finite-temperature molecular dynamics studies of lattice resistance in tantalum,"This manuscript explores the apparent discrepancy between experimental data and theoretical calculations of the lattice resistance of bcc tantalum. We present the first results for the temperature dependence of the Peierls stress in this system and the first ab initio calculation of the zero-temperature Peierls stress to employ periodic boundary conditions, which are those best suited to the study of metallic systems at the electron-structure level. Our ab initio value for the Peierls stress is over five times larger than current extrapolations of experimental lattice resistance to zero-temperature. Although we do find that the common techniques for such extrapolation indeed tend to underestimate the zero-temperature limit, the amount of the underestimation which we observe is only 10-20%, leaving open the possibility that mechanisms other than the simple Peierls stress are important in controlling the process of low temperature slip.",0212156v2 2003-02-21,Spin-Glass-like Transition and Hall Resistivity of Y2-xBixIr2O7,"Various physical properties of the pyrochlore oxide Y2-xBixIr2O7 have been studied. The magnetizations M measured under the conditions of the zero-field-cooling(ZFC) and the field-cooling(FC) have different values below the temperature T=TG. The anomalous T-dependence of the electrical resistivities r and the thermoelectric powers S observed at around TG indicates that the behavior of the magnetization is due to the transition to the state with the spin freezing. In this spin-frozen state, the Hall resistivities rH measured with the ZFC and FC conditions are found to have different values, too, in the low temperature phase (T=0.6.",0304423v2 2003-08-27,Room temperature domain wall pinning in bent ferromagnetic nanowires,"Mechanically bent nickel nanowires show clear features in their room temperature magnetoresistance when a domain wall is pinned at the location of the bend. By varying the direction of an applied magnetic field, the wire can be prepared either in a single-domain state or a two-domain state. The presence or absence of the domain wall acts to shift the switching fields of the nanowire. In addition, a comparison of the magnetoresistance of the nanowire with and without a domain wall shows a shift in the resistance correlated with the presence of a wall. The resistance is decreased by 20-30 milli-Ohms when a wall is present, compared to an overall resistance of 40-60 Ohms. A model of the magnetization was developed that allowed calculation of the magnetostatic energy of the nanowires, giving an estimate for the nucleation energy of a domain wall.",0308579v1 2003-11-27,Fabrication and Electrical Properties of Pure VO2 Phase Films,"We have grown VO2 thin films by laser ablation for electronic device applications. In obtaining the thin films of the pure VO2 phase, oxygen partial pressure is a critical parameter because vanadium oxides have several phases with the oxygen concentration. It is found that the pure VO2 films are epitaxially grown on Al2O3 substrate in the narrow ranges of 55-60 mTorr in an Ar+10% O2 ambient, and that the mixed phase films are synthesized when the deposition pressure slightly deviates from the optimum pressure. The (100) oriented VO2 films undergo an abrupt metal-insulator transition (MIT) with resistance change of an order of 104 at 338K. In the films of mixed phases, the small change of the resistance is observed at the same temperature. The polycrystalline films grown on SiO2/Si substrate undergo a broaden MIT of the resistance. Furthermore, the abrupt MIT and collective current motion appearing in metal are observed when the electric field is applied to the film.",0311616v2 2004-01-20,Non-Gaussian Resistance Noise near Electrical Breakdown in Granular Materials,"The distribution of resistance fluctuations of conducting thin films with granular structure near electrical breakdown is studied by numerical simulations. The film is modeled as a resistor network in a steady state determined by the competition between two biased processes, breaking and recovery. Systems of different sizes and with different levels of internal disorder are considered. Sharp deviations from a Gaussian distribution are found near breakdown and the effect increases with the degree of internal disorder. However, we show that in general this non-Gaussianity is related to the finite size of the system and vanishes in the large size limit. Nevertheless, near the critical point of the conductor-insulator transition, deviations from Gaussianity persist when the size is increased and the distribution of resistance fluctuations is well fitted by the universal Bramwell-Holdsworth-Pinton distribution.",0401352v1 2004-07-23,Thermal and Electrical Properties of gamma-NaxCoO2 (0.70 < x < 0.78),"We have performed specific heat and electric resistivity measurements of Na$_{x}$CoO$_{2}$ ($x=0.70$-0.78). Two anomalies have been observed in the specific heat data for $x=0.78$, corresponding to magnetic transitions at $T_{c}=22$ K and $T_{k}\simeq 9$ K reported previously. In the electrical resistivity, a steep decrease at $T_{c}$ and a bending-like variation at $T_{b}$(=120K for $x=0.78$) have been observed. Moreover, we have investigated the $x$-dependence of these parameters in detail. The physical properties of this system are very sensitive to $x$, and the inconsistent results of previous reports can be explained by a small difference in $x$. Furthermore, for a higher $x$ value, a phase separation into Na-rich and Na-poor domains occurs as we previously proposed, while for a lower $x$ value, from characteristic behaviors of the specific heat and the electrical resistivity at the low-temperature region, the system is expected to be in the vicinity of the magnetic instability which virtually exists below $x=0.70$.",0407614v1 2004-09-24,Hysteretic current-voltage characteristics and resistance switching at a rectifying Ti/Pr$_{0.7}$Ca$_{0.3}$MnO$_{3}$ interface,"We have characterized the vertical transport properties of epitaxial layered structures composed of Pr$_{0.7}$Ca$_{0.3}$MnO$_{3}$ (PCMO) sandwiched between SrRuO$_{3}$ (SRO) bottom electrode and several kinds of top electrodes such as SRO, Pt, Au, Ag, and Ti. Among the layered structures, Ti/PCMO/SRO is distinct due to a rectifying current-voltage ($I$--$V$) characteristic with a large hysteresis. Corresponding to the hysteresis of the $I$--$V$ characteristics, the contact resistance of the Ti/PCMO interface reversibly switches between two stable states by applying pulsed voltage stress. We propose a model for the resistance switching at the Ti/PCMO interface, in which the width and/or height of a Schottky-like barrier are altered by trapped charge carriers in the interface states.",0409657v1 2004-12-27,Depinning at the initial stage of the resistive transition in superconductors with a fractal cluster structure,"Depinning of vortices in percolative superconductor containing fractal clusters of a normal phase is considered. Transition of the superconductor into a resistive state corresponds to the percolation transition from a pinned vortex state to a resistive state when the vortices are free to move. The motion of the magnetic flux transferred by these vortices gives rise to the region of initial dissipation on current-voltage characteristic. The influence of normal phase clusters on distinctive features of current-voltage characteristics of percolative type-II superconductors is considered. It is found that an increase in the fractal dimension of the normal phase clusters causes the initial dissipation region to broaden out. The reason of this effect is an increase in the density of free vortices broken away from the pinning centers by the Lorentz force. Dependencies of the free vortex density on the fractal dimension of the normal phase cluster boundaries are obtained.",0412702v1 2005-04-20,Resistive relaxation in field-induced insulator-metal transition of a (La$_{0.4}$Pr$_{0.6}$)$_{1.2}$Sr$_{1.8}$Mn$_{2}$O$_{7}$ bilayer manganite single crystal,"We have investigated the resistive relaxation of a (La$_{0.4}$Pr$_{0.6}$)$_{1.2}$Sr$_{1.8}$Mn$_{2}$O$_{7}$ single crystal, in order to examine the slow dynamics of the field-induced insulator to metal transition of bilayered manganites. The temporal profiles observed in remanent resistance follow a stretched exponential function accompanied by a slow relaxation similar to that obtained in magnetization and magnetostriction data. We demonstrate that the remanent relaxation in magnetotransport has a close relationship with magnetic relaxation that can be understood in the framework of an effective medium approximation by assuming that the first order parameter is proportional to the second order one.",0504500v1 2005-05-19,Comparison of Measured and Calculated Specific Resistances of Pd/Pt Interfaces,"We compare specific resistances (AR equals area A times resistance R) of sputtered Pd/Pt interfaces measured in two different ways with no-free-parameter calculations. One way gives 2AR(Pd/Pt) of 0.29 (0.03) fohm-m(2) and the other 0.17 (0.13) fohm-m(2). From these we derive a best estimate of 2AR(Pd/Pt) of 0.28 (0.06) fohm-m(2), which overlaps with no-free-parameter calculations: 2AR(predicted) of 0.30 (0.04) fohm-m(2) for flat, perfect interfaces, or 0.33 (0.04) fohm-m(2) for interfaces composed of 2 monolayers of a 50percent-50percent PdPt alloy. These results support three prior examples of agreement between calculations and measurements for pairs of metals having the same crystal structure and the same lattice parameter to within 1 percent. We also estimate the spin-flipping probability at Pd/Pt interfaces as 0.13 (0.08).",0505488v2 2006-01-19,Spatially extended nature of resistive switching in perovskite oxide thin films,"We report the direct observation of the electric pulse induced resistance-change (EPIR) effect at the nano scale on La1-xSrxMnO3 (LSMO) thin films by the current measurement AFM technique. After a switching voltage of one polarity is applied across the sample by the AFM tip, the conductivity in a local nanometer region around the AFM tip is increased, and after a switching voltage of the opposite polarity is applied, the local conductivity is reduced. This reversible resistance switching effect is observed under both continuous and short pulse voltage switching conditions. It is important for future nanoscale non-volatile memory device applications.",0601451v1 2006-09-11,Imaging of Microscopic Sources of Resistive and Reactive Nonlinearities in Superconducting Microwave Devices,"The technique of low-temperature Laser Scanning Microscopy (LSM) has been applied to the investigation of local microwave properties in operating YBa2Cu3O7/LaAlO3 thin-film resonators patterned into a meandering strip transmission line. By using a modified newly developed procedure of spatially-resolved complex impedance partition, the influence of inhomogeneous current flow on the formation of nonlinear (NL) microwave response in such planar devices is analyzed in terms of the independent impact from resistive and inductive components. The modified procedure developed here is dramatically faster than our previous method. The LSM capability to probe the spatial variations of two-tone, third-order intermodulation currents on micron length scales is used to find the 2D distribution of the local sources of microwave NL. The results show that the dominant sources of microwave NL are strongly localized in the resistive domains.",0609244v1 2006-09-24,Swift-heavy-ion-irradiation-induced enhancement in electrical conductivity of chemical solution deposited La0.7Ba0.3MnO3 thin films,"Epitaxial thin films of La0.7Ba0.3MnO3 manganite, deposited using Chemical Solution Deposition technique, were irradiated by 200 MeV Ag+15 ions with a maximum ion dose up to 1x10^12 ions/cm2. Temperature- and magnetic field-dependent resistivity measurements on all the films (before and after irradiation) reveal a sustained decrease in resistivity with increasing ion dose. A maximum dose of 1x10^12 ions/cm2 suppresses resistivity by factors of 3 and 10, at 330 K [insulator-metal (I-M) transition] and at 10 K, respectively. On the other hand, with increasing ion dose, the magnetoresistance (MR) enhances in the vicinity of I-M transition but decreases at low temperatures. These results, corroborated by surface morphology of films, suggest that the origin of such properties lies in the irradiation induced improved crystallinity and epitaxial orientation, enhanced connectivity between grains, and conglomeration of grains which result in better conductivity at grain boundaries.",0609613v1 2006-10-06,Resistive hystersis effects in perovskite oxide-based heterostructure junctions,"In this paper, we report the electrical and structural properties of the oxide-based metal/ferroelectric/metal (MFM) junctions. The heterostructures are composed of ultrathin layers of La0.7Ca0.3MnO3 (LCMO) as a metallic layer and, BaTiO3 (BTO) as a ferroelectric layer. Junction based devices, having the dimensions of 400 x 200 micom2, have been fabricated upon LCMO/BTO/LCMO heterostructures by photolithography and Ar-ion milling technique. The DC current-voltage (I-V) characteristics of the MFM junctions were carried out. At 300 K, the devices showed the linear (I-V) characteristics, whereas at 77 K, (I-V) curves exhibited some reproducible switching behaviours with well-defined remnant currents. The resulting resistance modulation is very different from what was already reported in ultrathin ferroelectric layers displaying resistive switching. A model is presented to explain the datas",0610172v1 2007-02-26,Dielectrophoretically Assembled Polymer Nanowires for Gas Sensing,"We measured the electronic properties and gas sensing response of nanowires containing segments of poly(3,4-ethylenedioxythiophene)/poly(styrenesulfonate) (PEDOT/PSS) that were synthesized using anodic aluminum oxide (AAO) membranes. The nanowires have a ""striped"" structure of gold-PEDOT/PSS-gold and are typically 8 um long (1 um-6 um-1 um for each section, respectively) and 220 nm in diameter. Dielectrophoretic assembly was used to position single nanowires on pre-fabricated gold electrodes. A polymer conductivity of 11.5 +/- 0.7 S/cm and a contact resistance of 27.6 +/- 4 kOhm were inferred from resistance measurements of nanowires of varying length and diameter. When used as gas sensors, the wires showed a resistance change of 10.5%, 9%, and 4% at the saturation vapor pressure of acetone, methanol and ethanol, respectively. Sensor response and recovery were rapid (seconds) with excellent reproducibility in time and across devices. ""Striped"" template-grown nanowires are thus intriguing candidates for use in electronic nose vapor sensing systems.",0702619v1 2007-03-23,On the Kondo problem and thermodynamics of dilute magnetic alloys,"An argument is given showing that Coulomb attraction between conduction electrons and impurity ions in a dilute magnetic alloy (DMA) can be disregarded, provided the system's inverse temperature beta is replaced by an effective inverse temperature t < beta. This replacement allows to remove the singularity in Kondo's expression for DMA impurity resistivity and extend his theory to 0 K. The extended Kondo formula agrees with experimental data on resistivity of CuFe in the range of low temperatures and in the neighbourhood of the resistivity minimum. Using an asymptotic solution of the thermodynamics of a dilute s-d system at inverse temperature t, the impurity thermodynamic functions are derived and shown to provide good agreement with experimental data on CuFe, CuCr and (LaCe)Al_2 alloys in the low-temperature range. The magnitude of these functions agrees with experiment and does not require rescaling as in previous s-d theories. Nonlinear dependence of CuFe heat capacity on impurity concentration has been accounted for the first time.",0703617v1 2007-05-14,Scaling analysis of the magnetoresistance in Ga_{1-x}Mn_xAs,"We compare experimental resistivity data on Ga_{1-x}Mn_xAs films with theoretical calculations using a scaling theory for strongly disordered ferromagnets. All characteristic features of the temperature dependence of the resistivity can be quantitatively understood through this approach as originating from the close vicinity of the metal-insulator transition. In particular, we find that the magnetic field induced changes in resistance cannot be explained within a mean-field treatment of the magnetic state, and that accounting for thermal fluctuations is crucial for a quantitative analysis. Similarly, while the non-interacting scaling theory is in reasonable agreement with the data, we find clear evidence in favor of interaction effects at low temperatures.",0705.2016v2 2007-06-07,Meta-nematic transitions in a bilayer system: Application to the bilayer ruthenate,"It was suggested that the two consecutive metamagnetic transitions and the large residual resistivity discovered in Sr$_3$Ru$_2$O$_7$ can be understood via the nematic order and its domains in a single layer system. However, a recently reported anisotropy between two longitudinal resistivities induced by tilting the magnetic field away from the c-axis cannot be explained within the single layer nematic picture. To fill the gap in our understanding within the nematic order scenario, we investigate the effects of bilayer coupling and in-plane magnetic field on the electronic nematic phases in a bilayer system. We propose that the in-plane magnetic field in the bilayer system modifies the energetics of the domain formation, since it breaks the degeneracy of two different nematic orientations. Thus the system reveals a pure nematic phase with a resistivity anisotropy in the presence of an in-plane magnetic field. In addition to the nematic phase, the bilayer coupling opens a novel route to a hidden nematic phase that preserves the x-y symmetry of the Fermi surfaces.",0706.1069v3 2007-06-12,Graphene Spin Transistor,"Graphitic nanostructures, e.g. carbon nanotubes (CNT) and graphene, have been proposed as ideal materials for spin conduction[1-7]; they have long electronic mean free paths[8] and small spin-orbit coupling[9], hence are expected to have very long spin-scattering times. In addition, spin injection and detection in graphene opens new opportunities to study exotic electronic states such as the quantum Hall[10,11] and quantum spin Hall[9] states, and spin-polarized edge states[12] in graphene ribbons. Here we perform the first non-local four-probe experiments[13] on graphene contacted by ferromagnetic Permalloy electrodes. We observe sharp switching and often sign-reversal of the non-local resistance at the coercive field of the electrodes, indicating definitively the presence of a spin current between injector and detector. The non-local resistance changes magnitude and sign quasi-periodically with back-gate voltage, and Fabry-Perot-like oscillations[6,14,15] are observed, consistent with quantum-coherent transport. The non-local resistance signal can be observed up to at least T = 300 K.",0706.1597v1 2007-08-20,Negative magnetoresistance of ultra-narrow superconducting nanowires in the resistive state,"We present a phenomenological model qualitatively explaining negative magnetoresistance in quasi-one-dimensional superconducting channels in the resistive state. The model is based on the assumption that fluctuations of the order parameter (phase slips) are responsible for the finite effective resistance of a narrow superconducting wire sufficiently close to the critical temperature. Each fluctuation is accompanied by an instant formation of a quasi-normal region of the order of the non-equilibrium quasiparticle relaxation length 'pinned' to the core of the phase slip. The effective time-averaged voltage measured in experiment is a sum of two terms. First one is the conventional contribution linked to the rate of the fluctuations via the Josephson relation. Second term is the Ohmic contribution of this quasi-normal region. Depending on material properties of the wire, there might be a range of magnetic fields where the first term is not much affected, while the second term is effectively suppressed contributing to the experimentally observed negative magnetoresistance.",0708.2602v2 2007-11-23,Intrinsic and Extrinsic Performance Limits of Graphene Devices on SiO2,"The linear dispersion relation in graphene[1,2] gives rise to a surprising prediction: the resistivity due to isotropic scatterers (e.g. white-noise disorder[3] or phonons[4-8]) is independent of carrier density n. Here we show that acoustic phonon scattering[4-6] is indeed independent of n, and places an intrinsic limit on the resistivity in graphene of only 30 Ohm at room temperature (RT). At a technologically-relevant carrier density of 10^12 cm^-2, the mean free path for electron-acoustic phonon scattering is >2 microns, and the intrinsic mobility limit is 2x10^5 cm^2/Vs, exceeding the highest known inorganic semiconductor (InSb, ~7.7x10^4 cm^2/Vs[9]) and semiconducting carbon nanotubes (~1x10^5 cm^2/Vs[10]). We also show that extrinsic scattering by surface phonons of the SiO2 substrate[11,12] adds a strong temperature dependent resistivity above ~200 K[8], limiting the RT mobility to ~4x10^4 cm^2/Vs, pointing out the importance of substrate choice for graphene devices[13].",0711.3646v2 2008-02-11,Anomalous Hall effect in Fe/Cu bilayers,"The scaling of anomalous Hall resistivity on the longitudinal resistivity has been intensively studied in the different magnetic systems, including multilayers and granular films, to examine which mechanism, skew scattering or side-jump, dominates. The basis of the scaling law is that both the resistivities are due to the electron scattering at the imperfections in the materials. By studying of anomalous Hall effect (AHE) in the simple Fe/Cu bilayers, we demonstrate that the measured anomalous Hall effect should not follow the scaling laws derived from skew scattering or side-jump mechanism due to the short-circuit and shunting effects of the non-magnetic layers.",0802.1462v1 2008-04-09,Theory of a continuous Mott transition in two dimensions,"We study theoretically the zero temperature phase transition in two dimensions from a Fermi liquid to a paramagnetic Mott insulator with a spinon Fermi surface. We show that the approach to the bandwidth controlled Mott transition from the metallic side is accompanied by a vanishing quasiparticle residue and a diverging effective mass. The Landau parameters $F^0_s, F^0_a$ also diverge. Right at the quantum critical point there is a sharply defined `critical Fermi surface' but no Landau quasiparticle. The critical point has a $Tln\frac{1}{T}$ specific heat and a non-zero $T = 0$ resistivity. We predict an interesting {\em universal resistivity jump} in the residual resistivity at the critical point as the transition is approached from the metallic side. The crossovers out of the critical region are also studied. Remarkably the initial crossover out of criticality on the metallic side is to a Marginal Fermi Liquid metal. At much lower temperatures there is a further crossover into the Landau Fermi liquid. The ratio of the two crossover scales vanishes on approaching the critical point. Similar phenomena are found in the insulating side. The filling controlled Mott transition is also studied. Implications for experiments on the layered triangular lattice organic material $\kappa-(ET)_2Cu_2(CN)_3$ are discussed.",0804.1555v1 2008-04-28,Lattice Resistance to Dislocation Motion at the Nanoscale,"In this letter we propose a model that demonstrates the effect of free surface on the lattice resistance experienced by a moving dislocation in nanodimensional systems. This effect manifests in an enhanced velocity of dislocation due to the proximity of the dislocation line to the surface. To verify this finding, molecular dynamics simulations for an edge dislocation in bcc molybdenum are performed and the results are found to be in agreement with the numerical implementations of this model. The reduction in this effect at higher stresses and temperatures, as revealed by the simulations, confirms the role of lattice resistance behind the observed change in the dislocation velocity.",0804.4360v2 2008-05-13,The Role of Electrical and Thermal Contact Resistance for Joule Breakdown of Single-Wall Carbon Nanotubes,"Several data sets of electrical breakdown in air of single-wall carbon nanotubes (SWNTs) on insulating substrates are collected and analyzed. A universal scaling of the Joule breakdown power with nanotube length is found, which appears independent of the insulating substrates used or their thickness. This suggests the thermal resistances at the interface between SWNT and insulator, and between SWNT and electrodes, govern heat sinking from the nanotube. Analytical models for the breakdown power scaling are presented, providing an intuitive, physical understanding of the breakdown process. The electrical and thermal resistance at the electrode contacts limit the breakdown behavior for sub-micron SWNTs, the breakdown power scales linearly with length for microns-long tubes, and a minimum breakdown power (~ 0.05 uW) is observed for the intermediate (~ 0.5 um) length range.",0805.1937v1 2008-06-09,Transport properties and superconductivity in $Ba_{1-x}M_xFe_2As_2$ (M=La and K) with double FeAs layers,"We synthesized the samples $Ba_{1-x}M_xFe_2As_2$ (M=La and K) with $ThCr_2Si_2$-type structure. These samples were systematically characterized by resistivity, thermoelectic power (TEP) and Hall coefficient ($R_H$). $BaFe_2As_2$ shows an anomaly in resistivity at about 140 K. Substitution of La for Ba leads to a shift of the anomaly to low temperature, but no superconducting transition is observed. Potassium doping leads to suppression of the anomaly in resistivity and induces superconductivity at 38 K as reported by Rotter et al.\cite{rotter}. The Hall coefficient and TEP measurements indicate that the TEP is negative for $BaFe_2As_2$ and La-doped $BaFe_2As_2$, indicating n-type carrier; while potassium doping leads to change of the sign in $R_H$ and TEP. It definitely indicates p-type carrier in superconducting $Ba_{1-x}K_xFe_2As_2$ with double FeAs layers, being in contrast to the case of $LnO_{1-x}F_xFeAs$ with single FeAs layer. A similar superconductivity is also observed in the sample with nominal composition $Ba_{1-x}K_xOFe_2As_2$.",0806.1459v1 2009-02-21,Negative nonlocal resistance in mesoscopic gold Hall bars: Absence of giant spin Hall effect,"We report the observation of negative nonlocal resistances in multiterminal mesoscopic gold Hall bar structures whose characteristic dimensions are larger than the electron mean-free path. Our results can only be partially explained by a classical diffusive model of the nonlocal transport, and are not consistent with a recently proposed model based on spin Hall effects. Instead, our analysis suggests that a quasiballistic transport mechanism is responsible for the observed negative nonlocal resistance. Based on the sensitivity of our measurements and the spin Hall effect model, we find an upper limit for the spin Hall angle in gold of 0.022 at 4.5 K.",0902.3686v1 2009-08-26,Piezoresistance in chemically synthesized polypyrrole thin films,"The resistance of chemically synthesized polypyrrole (PPy) thin films is investigated as a function of the pressure of various gases as well as of the film thickness. A physical, piezoresistive response is found to coexist with a chemical response if the gas is chemically active, like, e.g., oxygen. The piezoresistance is studied separately by exposing the films to the chemically inert gases such as nitrogen and argon. We observe that the character of the piezoresistive response is a function not only of the film thickness, but also of the pressure. Films of a thickness below 70 nm show a decreasing resistance as pressure is applied, while for thicker films, the piezoresistance is positive. Moreover, in some films of thickness of about 70 nm, the piezoresistive response changes from negative to positive as the gas pressure is increased above 500 mbars. This behavior is interpreted in terms of a total piezoresistance which is composed of a surface and a bulk component, each of which contributes in a characteristic way. These results suggest that in polypyrrole, chemical sensing and piezoresistivity can coexist, which needs to be kept in mind when interpreting resistive responses of such sensors.",0908.3840v1 2009-09-28,The effects of superconductor-stabilizer interfacial resistance on quench of current-carrying coated conductor,"We present the results of numerical analysis of a model of normal zone propagation in coated conductors. The main emphasis is on the effects of increased contact resistance between the superconducting film and the stabilizer on the speed of normal zone propagation, the maximum temperature rise inside the normal zone, and the stability margins. We show that with increasing contact resistance the speed of normal zone propagation increases, the maximum temperature inside the normal zone decreases, and stability margins shrink. This may have an overall beneficial effect on quench protection quality of coated conductors. We also briefly discuss the propagation of solitons and development of the temperature modulation along the wire.",0909.5209v1 2009-11-02,Giant anomalous Hall resistivity of the room temperature ferromagnet Fe3Sn2 - a frustrated metal with the kagome-bilayer structure,"We have investigated magnetic and transport properties of the {\it kagom\'{e}-bilayer} ferromagnet Fe$_{3}$Sn$_{2}$. A soft ferromagnetism and a large anomalous Hall effect are observed. The saturated Hall resistivity of Fe$_{3}$Sn$_{2}$ is 3.2 $\mu\Omega$cm at 300 K, which is almost 20 times higher than that of typical itinerant-ferromagnets such as Fe and Ni. The anomalous Hall coefficient $R_{{\rm s}}$ is 6.7$\times10^{-9}$ $\Omega$cm/G at 300 K, which is three orders of magnitude larger than that of pure Fe. $R_{{\rm s}}$ obeys an unconventional scaling to the longitudinal resistivity, $\rho_{xx}$, of $R_{{\rm s}} \propto \rho_{xx}^{3.3}$. Such a relationship cannot be explained by the skew and/or side-jump mechanisms and indicates that the origin of the anomalous Hall effect in the frustrated magnet Fe$_{3}$Sn$_{2}$ is indeed extraordinary.",0911.0289v1 2010-04-19,Towards a Quantitative Description of Solid Electrolyte Conductance Switches,"We present a quantitative analysis of the steady state electronic transport in a resistive switching device. The device is composed of a thin film of Ag$_{2}$S (solid electrolyte) contacted by a Pt nano-contact acting as ion-blocking electrode, and a large area Ag reference electrode. When applying a bias voltage both ionic and electronic transport occurs, and depending on the polarity it causes an accumulation of ions around the nano-contact. At small applied voltages (pre-switching) we observed this as a strongly nonlinear current-voltage curve, which have been modeled using the Hebb-Wagner treatment for polarization of a mixed conductor. This model correctly describes the transport of the electrons within the polarized solid electrolyte in the steady state up until the resistance switching, covering the entire range of non-stoichiometries, and including the supersaturation range just before the deposition of elemental silver. In this way, it is a step towards a quantitative understanding of the processes that lead to resistance switching.",1004.3079v1 2010-05-18,A general figure of merit for thick and thin transparent conductive carbon nanotube coatings,"We suggest a wavelength-dependent figure of merit for transparent conducting nanotube networks, composed of the sheet resistance and the optical density. We argue that this would be more useful than other suggestions prevailing in the literature, because it relies on more realistic assumptions regarding the optical parameters of real nanotubes: it takes into account the fact that the dc resistivity depends on the concentration of free carriers, while the visible absorption is caused by bound carriers. Based on sheet resistance measurements and wide-range transmission spectra, we compare several commercial nanotube types and find correlation between metal enrichment and figure of merit. A simple graphical approach is suggested to determine if the required optical and transport properties can be achieved by varying the thickness of the nanotube layer or a more aggressive treatment is needed. The procedure can be extended to oxide coatings as well.",1005.3125v1 2010-05-30,On the Corrosion Resistance of Porous Electroplated Zinc Coatings in Different Corrosive Media,"The corrosion resistance of an electroplated (EP) Zn coating whose surface was chemically etched to produce surface defects (pores) is investigated in this work. Impedance and DC polarisation measururements were employed to study the behaviour of such coating in various corrosive media (NaCl, NaOH and rain water). Four different faradaic relaxation processes were clearly revealed in different NaCl concentrations (from 0.1M to 1M). In the most concentrated solutions at least three relaxation processes at low frequencies (LF) appeared and were related to zinc deposition and dissolution. At lower concentrations and depending on the pH, only one process was observed. The charge transfer resistance (Rct) and the corrosion current (Icorr) were practically stable in the pH range 5 to 10. In deaerated NaCl 0.1M, the EIS diagrams showed two time-constants at very close frequencies. From the EIS diagrams the porous nature of the coating was highlighted and showed that the dissolution mechanisms occurred at the base of the pores.",1005.5554v1 2010-06-12,Ex-situ Tunnel Junction Process Technique Characterized by Coulomb Blockade Thermometry,"We investigate a wafer scale tunnel junction fabrication method, where a plasma etched via through a dielectric layer covering bottom Al electrode defines the tunnel junction area. The ex-situ tunnel barrier is formed by oxidation of the bottom electrode in the junction area. Room temperature resistance mapping over a 150 mm wafer give local deviation values of the tunnel junction resistance that fall below 7.5 % with an average of 1.3 %. The deviation is further investigated by sub-1 K measurements of a device, which has one tunnel junction connected to four arrays consisting of N junctions (N = 41, junction diameter 700 nm). The differential conductance is measured in single-junction and array Coulomb blockade thermometer operation modes. By fitting the experimental data to the theoretical models we found an upper limit for the local tunnel junction resistance deviation of ~5 % for the array of 2N+1 junctions. This value is of the same order as the minimum detectable deviation defined by the accuracy of our experimental setup.",1006.2436v1 2010-08-24,"Magnetism of mixed quaternary Heusler alloys: (Ni,T)$_{2}$MnSn (T=Cu,Pd) as a case study","The electronic properties, exchange interactions, finite-temperature magnetism, and transport properties of random quaternary Heusler Ni$_{2}$MnSn alloys doped with Cu- and Pd-atoms are studied theoretically by means of {\it ab initio} calculations over the entire range of dopant concentrations. While the magnetic moments are only weakly dependent on the alloy composition, the Curie temperatures exhibit strongly non-linear behavior with respect to Cu-doping in contrast with an almost linear concentration dependence in the case of Pd-doping. The present parameter-free theory agrees qualitatively and also reasonably well quantitatively with the available experimental results. An analysis of exchange interactions is provided for a deeper understanding of the problem. The dopant atoms perturb electronic structure close to the Fermi energy only weakly and the residual resistivity thus obeys a simple Nordheim rule. The dominating contribution to the temperature-dependent resistivity is due to thermodynamical fluctuations originating from the spin-disorder, which, according to our calculations, can be described successfully via the disordered local moments model. Results based on this model agree fairly well with the measured values of spin-disorder induced resistivity.",1008.4060v1 2010-10-29,Nd induced Mn spin-reorientation transition in NdMnAsO,"A combination of synchrotron X-ray, neutron powder diffraction, magnetization, heat capacity and electrical resistivity measurements reveals that NdMnAsO is an antiferromagnetic semiconductor with large Neel temperature (TN = 359(2) K). At room temperature the magnetic propagation vector k = 0 and the Mn moments are directed along the crystallographic c-axis (mMn = 2.41(6) BM). Upon cooling a spin reorientation (SR) transition of the Mn moments into the ab-plane occurs (TSR = 23 K). This coincides with the long range ordering of the Nd moments, which are restricted to the basal plane. The magnetic propagation vector remains k = 0. At base temperature (1.6 K) the fitted moments are mab,Mn = 3.72(1) BM and mab,Nd = 1.94(1) BM. The electrical resistivity is characterized by a broad maximum at 250 K, below which it has a metallic temperature dependence but semiconducting magnitude (rho250K = 50 Ohm cm, residual resistivity ratio = 2), and a slight upturn at the SR transition.",1010.6145v1 2010-11-04,Electron interaction-driven insulating ground state in Bi2Se3 topological insulators in the two dimensional limit,"We report a transport study of ultrathin Bi2Se3 topological insulators with thickness from one quintuple layer to six quintuple layers grown by molecular beam epitaxy. At low temperatures, the film resistance increases logarithmically with decreasing temperature, revealing an insulating ground state. The sharp increase of resistance with magnetic field, however, indicates the existence of weak antilocalization, which should reduce the resistance as temperature decreases. We show that these apparently contradictory behaviors can be understood by considering the electron interaction effect, which plays a crucial role in determining the electronic ground state of topological insulators in the two dimensional limit.",1011.1055v1 2011-02-03,Temperature dependent resistivity in bilayer graphene due to flexural phonons,"We have studied electron scattering by out-of-plane (flexural) phonons in doped suspended bilayer graphene. We have found the bilayer membrane to follow the qualitative behavior of the monolayer cousin. In the bilayer, different electronic structure combine with different electron-phonon coupling to give the same parametric dependence in resistivity, and in particular the same temperature $T$ behavior. In parallel with the single layer, flexural phonons dominate the phonon contribution to resistivity in the absence of strain, where a density independent mobility is obtained. This contribution is strongly suppressed by tension, and in-plane phonons become the dominant contribution in strained samples. Among the quantitative differences an important one has been identified: room $T$ mobility in bilayer graphene is substantially higher than in monolayer. The origin of quantitative differences has been unveiled.",1102.0807v1 2011-05-19,Anisotropic in-plane resistivity in the nematic phase of the iron pnictides,"We show that the interference between scattering by impurities and by critical spin fluctuations gives rise to anisotropic transport in the Ising-nematic state of the iron pnictides. The effect is closely related to the non-Fermi liquid behavior of the resistivity near an antiferromagnetic quantum critical point. Our theory not only explains the observed sign of the resistivity anisotropy $\Delta\rho$ in electron doped systems, but also predicts a sign change of $\Delta\rho$ upon sufficient hole doping. Furthermore, our model naturally addresses the changes in $\Delta\rho$ upon sample annealing and alkaline-earth substitution.",1105.3906v2 2011-08-17,Control of rectifying and resistive switching behavior in BiFeO3 thin films,"BiFeO3 thin films have been grown on Pt/Ti/SiO2/Si substrates with pulsed laser deposition using Au as the top electrode. The resistive switching property of the Au/BiFeO3/Pt stack has been significantly improved by carefully tuning the oxygen pressure during the growth, and a large switching ratio of ~4500 has been achieved. The deposition pressure modifies the concentration of oxygen vacancies and the rectifying behavior of the Au/BiFeO3 junction, and consequently influences the resistive switching behavior of the whole stack. The switching takes place homogeneously over the entire electrode, and shows a long-term retention.",1108.3454v1 2011-09-05,The direct relation between the coefficient of the low temperature resistivity T^2 term and the superconducting transition temperature Tc,"In several superconductors above the superconducting transition temperature Tc, the electrical resistivity is of the form {\rho} =AT^2. We show that there exists an empirical relation between Tc and A when both vary with an external parameter, e.g. pressure. The more resistive the sample the higher the Tc. Landau theory shows that it is a general feature of Fermi Liquids, as {\rho} is governed by the scattering that bounds the pairs condensing at Tc. We develop a method that allows the determination of the coupling constant {\lambda} that is validated when used to the transport properties of superfluid 3He.",1109.0853v1 2011-10-17,In Situ Imaging of the Conducting Filament in a Silicon Oxide Resistive Switch,"The nature of the conducting filaments in many resistive switching systems has been elusive. Through in situ transmission electron microscopy, we image the real-time formation and evolution of the filament in a silicon oxide resistive switch. The electroforming process is revealed to involve the local enrichment of silicon from the silicon oxide matrix. Semi-metallic silicon nanocrystals with structural variations from the conventional diamond cubic form of silicon are observed, which likely accounts for the conduction in the filament. The growth and shrinkage of the silicon nanocrystals in response to different electrical stimuli show energetically viable transition processes in the silicon forms, offering evidence to the switching mechanism. The study here also provides insights into the electrical breakdown process in silicon oxide layers, which are ubiquitous in a host of electronic devices.",1110.3755v1 2011-12-02,Wigner-Mott scaling of transport near the two-dimensional metal-insulator transition,"Electron-electron scattering usually dominates the transport in strongly correlated materials. It typically leads to pronounced resistivity maxima in the incoherent regime around the coherence temperature $T^{*}$, reflecting the tendency of carriers to undergo Mott localization following the demise of the Fermi liquid. This behavior is best pronounced in the vicinity of interaction-driven (Mott-like) metal-insulator transitions, where the $T^{*}$ decreases, while the resistivity maximum $\rho_{max}$ increases. Here we show that, in this regime, the entire family of resistivity curves displays a characteristic scaling behavior $\rho(T)/\rho_{max}\approx F(T/T_{max}),$ while the $\rho_{max}$ and $T_{max}\sim T^{*}$ assume a powerlaw dependence on the quasi-particle effective mass $m^{*}$. Remarkably, precisely such trends are found from an appropriate scaling analysis of experimental data obtained from diluted two-dimensional electron gases in zero magnetic fields. Our analysis provides strong evidence that inelastic electron-electron scattering -- and not disorder effects -- dominates finite temperature transport in these systems, validating the Wigner-Mott picture of the two-dimensional metal-insulator transition.",1112.0440v2 2012-02-15,Non-linear resistivity and heat dissipation in monolayer graphene,"We have experimentally studied the nonlinear nature of electrical conduction in monolayer graphene devices on silica substrates. This nonlinearity manifests itself as a nonmonotonic dependence of the differential resistance on applied DC voltage bias across the sample. At temperatures below ~70K, the differential resistance exhibits a peak near zero bias that can be attributed to self-heating of the charge carriers. We show that the shape of this peak arises from a combination of different energy dissipation mechanisms of the carriers. The energy dissipation at higher carrier temperatures depends critically on the length of the sample. For samples longer than 10um the heat loss is shown to be determined by optical phonons at the silica-graphene interface.",1202.3394v1 2012-04-19,Observation of Negative Contact Resistances in Graphene Field-Effect Transistors,"The gate-voltage (VG) dependence of the contact resistance (RC) in graphene field-effect transistors is characterized by the transmission line model. The RC-VG characteristics of Ag, Cu, and Au contacts display a dip around the charge neutrality point, and become even negative with Ag contacts. The dip structure is well reproduced by a model calculation that considers a metal-contact-induced potential variation near the metal contact edges. The apparently negative RC originates with the carrier doping from the metal contacts to the graphene channel and appears when the doping effect is more substantial than the actual contact resistance precisely at the contacts. The negative RC can appear at the metal contacts to Dirac-cone systems such as graphene.",1204.4315v2 2012-05-24,Intrinsic Electron-Phonon Resistivity in Bi2Se3 in the Topological Regime,"We measure the temperature-dependent carrier density and resistivity of the topological surface state of thin exfoliated Bi2Se3 in the absence of bulk conduction. When the gate-tuned chemical potential is near or below the Dirac point the carrier density is strongly temperature dependent reflecting thermal activation from the nearby bulk valence band, while above the Dirac point, unipolar n-type surface conduction is observed with negligible thermal activation of bulk carriers. In this regime linear resistivity vs. temperature reflects intrinsic electron-acoustic phonon scattering. Quantitative comparison with a theoretical transport calculation including both phonon and disorder effects gives the ratio of deformation potential to Fermi velocity D/\hbarvF = 4.7 {\AA}-1. This strong phonon scattering in the Bi2Se3 surface state gives intrinsic limits for the conductivity and charge carrier mobility at room temperature of ~550 {\mu}S per surface and ~10,000 cm2/Vs.",1205.5554v2 2012-07-21,Simulation of magnetoresistance in disordered ultracold atomic Bose gases,"Anderson localization was first investigated in the context of electrons in solids. One of the successes was in explaining the puzzle of negative magneto-resistance - as early as the 1940s it had been observed that electron diffusion rates in some materials can increase with the application of a magnetic field. Anderson localization has now been demonstrated in ultra-cold atomic gases. We present a theoretical study of the two-dimensional ultra-cold Bose gas in the presence of disorder, to which we apply a synthetic magnetic field. We demonstrate that, in the ballistic transport regime this leads to positive magneto-resistance and that, in the diffusive and strong localization regimes, can also lead to negative magneto-resistance. We propose experimental scenarios to observe these effects.",1207.5095v1 2012-07-26,Spin-orbit-coupling induced domain-wall resistance in diffusive ferromagnets,"We investigate diffusive transport through a number of domain wall (DW) profiles of the important magnetic alloy Permalloy taking into account simultaneously noncollinearity, alloy disorder, and spin-orbit coupling fully quantum mechanically, from first principles. In addition to observing the known effects of magnetization mistracking and anisotropic magnetoresistance, we discover a not-previously identified contribution to the resistance of a DW that comes from spin-orbit-coupling-mediated spin-flip scattering in a textured diffusive ferromagnet. This adiabatic DW resistance, which should exist in all diffusive DWs, can be observed by varying the DW width in a systematic fashion in suitably designed nanowires.",1207.6277v2 2012-08-01,Textured Superconductivity in the Presence of a Coexisting Order: Ce115s and Other Heavy-Fermion Compounds,"Superconductivity in strongly correlated electron systems frequently emerges in proximity to another broken symmetry. In heavy-electron superconductors, the nearby ordered state most commonly is magnetism, and the so-called Ce115 heavy-electron compounds have been particularly instructive for revealing new relationships between magnetism and superconductivity. From measurements of the resistive and bulk transitions to superconductivity in these materials, we find that the resistive transition appears at a temperature considerably higher than the bulk transition when superconductivity and magnetic order coexist, but this temperature difference disappears in the absence of long-range magnetic order. Further, in the pressure-temperature region of coexistence in CeRhIn5, a new anisotropy in the resistive transition develops even though the tetragonal crystal structure apparently remains unchanged, implying a form of textured superconductivity. We suggest that this texture may be a generic response to coexisting order in these and other heavy-fermion superconductors.",1208.0253v1 2012-09-20,Surface resistance measurements of HTS thin films using SLAO dielectric resonator,"Surface resistance of HTS films is typically measured using Sapphire dielectric rod resonators enclosed in a copper cavity. In this paper we present surface resistance measurements of YBa2Cu3O7-{\delta} films using Strontium Lanthanum Aluminate (SLAO) at a resonant frequency of 18.2 GHz. We have performed the error analysis of the cavity loaded with SLAO dielectric rod and also verification measurements using two Sapphire (Al2O3) rod resonators operating at resonant frequencies of 24.6 GHz and 10 GHz respectively. Good agreement between the values of Rs of two sets of YBa2Cu3O7-{\delta} films measured using the SLAO and the Sapphire dielectrics has been obtained after a frequency scaling of Rs was applied. Using different dielectric rods of the same size in the same cavity for measurements of Rs of HTS films, it is feasible to do microwave characterization of the same films at differing frequencies.",1209.4519v1 2012-12-04,UV/Ozone treatment to reduce metal-graphene contact resistance,"We report reduced contact resistance of single-layer graphene devices by using ultraviolet ozone (UVO) treatment to modify the metal/graphene contact interface. The devices were fabricated from mechanically transferred, chemical vapor deposition (CVD) grown, single layer graphene. UVO treatment of graphene in the contact regions as defined by photolithography and prior to metal deposition was found to reduce interface contamination originating from incomplete removal of poly(methyl methacrylate) (PMMA) and photoresist. Our control experiment shows that exposure times up to 10 minutes did not introduce significant disorder in the graphene as characterized by Raman spectroscopy. By using the described approach, contact resistance of less than 200 {\Omega} {\mu}m was achieved, while not significantly altering the electrical properties of the graphene channel region of devices.",1212.0838v1 2013-03-25,Kinetics of excitations on the Fermi arcs in underdoped cuprates at low temperature,"The Fermi-liquid-like (FL) resistivity recently observed in clean HgBa2CuO4 below the pseudogap temperature was related to carriers at the nodal points on the Fermi surface [4]. We show that this necessitates important implications for the electronic spectrum of underdoped (UD) cuprates in whole. Photoemission experiments picture the spectrum as of metallic arcs separated from each other by regions with large energy gaps. We solved the kinetic equation in such model rigorously. The Fermi arcs carriers contribute to FL resistivity, if scattering between the opposite nodal points admits the Umklapp processes. The Hall coefficient defines the effective number of carriers on arcs and has the positive sign. For clean materials the expression is applicable only at weak magnetic fields. We discuss the Fermi arcs concept further in light of recent experimental findings and argue that the idea of reconstructed FS in UD cuprates is not consistent with the FL-like resistivity.",1303.6252v2 2013-03-27,First-Principles Calculation of Thermal Transport in the Metal/Graphene System,"Thermal properties in the metal/graphene (Gr) systems are analyzed by using an atomistic phonon transport model based on Landauer formalism and first-principles calculations. The specific structures under investigation include chemisorbed Ni(111)/Gr, physisorbed Cu(111)/Gr and Au(111)/Gr, as well as Pd(111)/Gr with intermediate characteristics. Calculated results illustrate a strong dependence of thermal transfer on the details of interfacial microstructures. In particular, it is shown that the chemisorbed case provides a generally smaller interfacial thermal resistance than the physisorbed due to the stronger bonding. However, our calculation also indicates that the weakly chemisorbed interface of Pd/Gr may be an exception, with the largest thermal resistance among the considered. Further examination of the electrostatic potential and interatomic force constants reveal that the mixed bonding force between the Pd and C atoms results in incomplete hybridization of Pd and graphene orbital states at the junction, leading effectively to two phonon interfaces and a larger than expected thermal resistance. Comparison with available experimental data shows good agreement. The result clearly suggests the feasibility of phonon engineering for thermal property optimization at the interface.",1303.6936v1 2013-05-22,Electron Transport Through Ag-Silicene-Ag Junctions,"For several years the electronic structure properties of the novel two-dimensional system silicene have been studied extensively. Electron transport across metal-silicence junctions, however, remains relatively unexplored. To address this issue, we developed and implemented a theoretical framework that utilizes the tight-binding Fisher-Lee relation to span non-equilibrium Green's function (NEGF) techniques, the scattering method, and semiclassical Boltzmann transport theory. Within this hybrid quantum-classical, two-scale framework, we calculated transmission and reflection coefficients of monolayer and bilayer Ag-silicene-Ag junctions using the NEGF method in conjunction with density functional theory; derived and calculated the group velocities; and computed resistance using the semi-classical Boltzmann equation. We found that resistances of these junctions are $\sim${}$ 0.08 \fom$ for monolayer silicene junctions and $\sim${}$ 0.3 \fom$ for bilayer ones, factors of $\sim$8 and $\sim$2, respectively, smaller than Sharvin resistances estimated via the Landauer formalism.",1305.5285v1 2013-06-13,"Investigation of the quaternary Fe2-xCoxMnSi alloys by structural, magnetic, resistivity and spin polarization measurements","Effects of the Co substitution have been observed on the structural, magnetic and magneto-transport properties of Fe2-xCoxMnSi alloy. Curie temperature (TC) and saturation magnetization (MS) of these alloys increased linearly with the Co substitution. Competitive magnetic interaction between ferromagnetic (FM) and anti-ferromagnetic (AFM) phases exists in Fe2-xCoxMnSi for x less than 0.2, AFM phase is completely disappears for x greater than or equal to 0.2. The value of Rhodes-Wohlfarth ratio pc/ps is greater than one for these alloys which is the characteristics of iterant magnetism present in the system. M\""ossbauer spectroscopic measurements have been done to investigate the atomic disorder and local magnetic moment for some x values. Resistivity measurements also confirm the stability of ferromagnetism with the concentration of Co and also show a sign of half metallicity. Resistivity shows semiconducting behaviour for x = 0.4 which is interesting in view of spin gapless semiconductors.",1306.3086v3 2013-06-21,Carrier density modulation in graphene underneath Ni electrode,"We investigate the transport properties of graphene underneath metal to reveal whether the carrier density in graphene underneath source/drain electrodes in graphene field-effect transistors is fixed. The resistance of the graphene/Ni double-layered structure has shown a graphene-like back-gate bias dependence. In other words, the electrical properties of graphene are not significantly affected by its contact with Ni. This unexpected result may be ascribed to resist residuals at the metal/graphene interface, which may reduce the interaction between graphene and metals. In a back-gate device fabricated using the conventional lithography technique with an organic resist, the carrier density modulation in the graphene underneath the metal electrodes should be considered when discussing the metal/graphene contact.",1306.5086v1 2013-07-29,Molecular Doping of Multilayer MoS2 Field-effect Transistors: Reduction in Sheet and Contact Resistances,"For the first time, polyethyleneimine (PEI) doping on multilayer MoS2 field-effect transistors are investigated. A 2.6 times reduction in sheet resistance, and 1.2 times reduction in contact resistance have been achieved. The enhanced electrical characteristics are also reflected in a 70% improvement in ON current, and 50% improvement in extrinsic field-effect mobility. The threshold voltage also confirms a negative shift upon the molecular doping. All studies demonstrate the feasibility of PEI molecular doping in MoS2 transistors, and its potential applications in layer-structured semiconducting 2D crystals.",1307.7643v2 2013-09-15,Large lattice distortions associated with the magnetic transition in La0.7Sr0.3MnO3,"Colossal magnetoresistance (CMR) is associated with the phase transition from a metallic ferromagnetic to insulating paramagnetic phase, which can be controlled by an applied magnetic field. The insulating phase occurs due to trapping of the charge carriers by polaronic lattice distortions, which raise the resistivity. Theories based on local physics predict that the magnitude of the resistivity jump at Tc is determined by how much, on average, the amplitude of these distortions increases at the phase transition. Using neutron scattering, we measured the average distortion amplitude in La0.7Sr0.3MnO3. Surprisingly, its increase from below to above Tc is just as large as in other manganites, which have a much larger resistivity jump. This result suggests that the strength of CMR is determined not by the size of distortions, but by their cooperative nature specific to each compound. Existing theories need to be extended to include correlations between different unit cells to explain and predict the strength of CMR.",1309.3747v1 2013-09-20,Surface-resistance measurements using superconducting stripline resonators,"We present a method to measure the absolute surface resistance of conductive samples at a set of GHz frequencies with superconducting lead stripline resonators at temperatures 1- 6K. The stripline structure can easily be applied for bulk samples and allows direct calculation of the surface resistance without the requirement of additional calibration measurements or sample reference points. We further describe a correction method to reduce experimental background on high-Q resonance modes by exploiting TEM-properties of the external cabling. We then show applications of this method to the reference materials gold, tantalum, and tin, which include the anomalous skin effect and conventional superconductivity. Furthermore, we extract the complex optical conductivity for an all-lead stripline resonator to find a coherence peak and the superconducting gap of lead.",1309.5331v2 2013-10-17,The Influence of Ca and Y on the Microstructure and Corrosion Resistance of Vacuum Die Casting AZ91 Alloy,"The influence of Ca and Y on the microstructure and corrosion resistance of vacuum die casting AZ91 alloy is investigated using optical microscope, electron scanning microscope, weight-loss test and electrochemical corrosion test. The results indicate that the microstructure of AZ91 alloy can be refined, amount of Mg17Al12 phases is reduced, making Mg17Al12 phases transform from banding to reticular, and stringer Al2Ca phases and block Al2Y phases are formed through adding both Ca and Y. The corrosion resistance of AZ91 magnesium alloy can be increased greatly by adding both Ca and Y. The corrosion rate of AZ91-1.5Ca-1.0Y alloy is dropped to 16.2% of that of AZ91 alloy immersed in 3.5% NaCl aqueous solution for 24 hours. The corrosion current density of AZ91-1.5Ca-1.0Y alloy is dropped by one order of magnitude.",1310.4671v1 2013-11-05,Effect of disorder on the resistivity anisotropy near the electronic nematic phase transition in pure and electron-doped BaFe$_2$As$_2$,"We show that the strain-induced resistivity anisotropy in the tetragonal state of the representative underdoped Fe-arsenides BaFe$_2$As$_2$, Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ and Ba(Fe$_{1-x}$Ni$_x$)$_2$As$_2$ is independent of disorder over a wide range of defect and impurity concentrations. This result demonstrates that the anisotropy in the in-plane resistivity in the paramagnetic orthorhombic state of this material is not due to elastic scattering from anisotropic defects, and is most easily understood in terms of an intrinsic anisotropy in the electronic structure.",1311.0933v2 2013-11-14,Mechanically Modulated Tunneling Resistance in Monolayer MoS2,"We report on the modulation of tunneling resistance in MoS2 monolayers by nano-indentation using an atomic force microscope (AFM). The resistance between the conductive AFM tip and the bottom electrode separated by a monolayer MoS2 is reversibly reduced by up to 4 orders of magnitude, which is attributed to enhanced quantum tunneling when the monolayer is compressed by the tip force. Under the WKB approximation, the experimental data is quantitatively explained by using the metal-insulator-metal tunneling diode model. As an ideal tunneling medium, the defect-free, nanometer-thick MoS2 monolayer can serve as the active layer for non-impacting nano-electro-mechanical switches.",1311.3608v1 2014-03-21,MoS2 Field-effect Transistors with Graphene/Metal Heterocontacts,"For the first time, n-type few-layer MoS2 field-effect transistors with graphene/Ti as the hetero-contacts have been fabricated, showing more than 160 mA/mm drain current at 1 {\mu}m gate length with an on-off current ratio of 107. The enhanced electrical characteristic is confirmed in a nearly 2.1 times improvement in on-resistance and a 3.3 times improvement in contact resistance with hetero-contacts compared to the MoS2 FETs without graphene contact layer. Temperature dependent study on MoS2/graphene hetero-contacts has been also performed, still unveiling its Schottky contact nature. Transfer length method and a devised I-V method have been introduced to study the contact resistance and Schottky barrier height in MoS2/graphene /metal hetero-contacts structure.",1403.5485v2 2014-07-09,Thermal transport properties of metal/MoS2 interfaces from first principles,"Thermal transport properties at the metal/MoS2 interfaces are analyzed by using an atomistic phonon transport model based on the Landauer formalism and first-principles calculations. The considered structures include chemisorbed Sc(0001)/MoS2 and Ru(0001)/MoS2, physisorbed Au(111)/MoS2, as well as Pd(111)/MoS2 with intermediate characteristics. Calculated results illustrate a distinctive dependence of thermal transfer on the details of interfacial microstructures. More specifically, the chemisorbed case with a stronger bonding exhibits a generally smaller interfacial thermal resistance than the physisorbed. Comparison between metal/MoS2 and metal/graphene systems suggests that metal/MoS2 is significantly more resistive. Further examination of lattice dynamics identifies the presence of multiple distinct atomic planes and bonding patterns at the interface as the key origin of the observed large thermal resistance.",1407.2335v1 2014-10-30,Highly resistive epitaxial Mg-doped GdN thin films,"We report the growth by molecular beam epitaxy of highly resistive GdN, using intentional doping with magnesium. Mg-doped GdN layers with resistivities of 1000 {\Omega}.cm and carrier concentrations of 10E16 cm-3 are obtained for films with Mg concentrations up to 5 x 10E19 atoms/cm3. X-ray diffraction rocking curves indicate that Mg-doped GdN films have crystalline quality very similar to undoped GdN films, showing that the Mg doping did not affect the structural properties of the films. A decrease of the Curie temperature with decreasing the electron density is observed, supporting a recently suggested magnetic polaron scenario [F. Natali et al., Phys. Rev. B 87, 035202 (2013)].",1410.8228v1 2014-11-12,Probing a spin-glass state in SrRuO3 thin films through higher-order statistics of resistance fluctuations,"The complex perovskite oxide SrRuO3 shows intriguing transport properties at low temperatures due to the interplay of spin, charge, and orbital degrees of freedom. One of the open questions in this system is regarding the origin and nature of the low-temperature glassy state. In this paper we report on measurements of higher-order statistics of resistance fluctuations performed in epitaxial thin films of SrRuO3 to probe this issue. We observe large low-frequency non-Gaussian resistance fluctuations over a certain temperature range. Our observations are compatible with that of a spin-glass system with properties described by hierarchical dynamics rather than with that of a simple ferromagnet with a large coercivity.",1411.3101v1 2014-12-02,On the field dependent surface resistance of niobium on copper cavities,"The surface resistance Rs of superconducting cavities prepared by sputter coating a thin niobium film on a copper substrate increases significantly stronger with the applied RF field compared to cavities of bulk material. A possible cause is that due to the thermal boundary resistance between the copper substrate and the niobium film Rs is enhanced due to global heating of the inner cavity wall. Introducing helium gas in the cavity and measuring its pressure as a function of applied field allowed to conclude that the inner surface of the cavity is heated up by only 60+/-60 mK when Rs increases with Eacc by 100 nOhm. This is more than one order of magnitude less than what one would expect from global heating. Additionally the effect of cooldown speed and low temperature baking have been investigated in the framework of these experiments. It is shown that for current state of the art niobium on copper cavities there is only a detrimental effect of low temperature baking. A fast cooldown results in a lowered Rs.",1412.0892v1 2015-01-20,Generation and detection of pure valley current by electrically induced Berry curvature in bilayer graphene,"Valley is a useful degree of freedom for non-dissipative electronics since valley current that can flow even in an insulating material does not accompany electronic current. We use dual-gated bilayer graphene in the Hall bar geometry to electrically control broken inversion symmetry or Berry curvature as well as the carrier density to generate and detect the pure valley current. We find a large nonlocal resistance and a cubic scaling between the nonlocal resistance and the local resistivity in the insulating regime at zero-magnetic field and 70 K as evidence of the pure valley current. The electrical control of the valley current in the limit of zero conductivity allows non-dissipative induction of valley current from electric field and thus provides a significant contribution to the advancement of non-dissipative electronics.",1501.04776v1 2015-02-24,Unidirectional spin Hall magnetoresistance in ferromagnet/normal metal bilayers,"Magnetoresistive effects are usually invariant upon inversion of the magnetization direction. In noncentrosymmetric conductors, however, nonlinear resistive terms can give rise to a current dependence that is quadratic in the applied voltage and linear in the magnetization. Here we demonstrate that such conditions are realized in simple bilayer metal films where the spin-orbit interaction and spin-dependent scattering couple the current-induced spin accumulation to the electrical conductivity. We show that the longitudinal resistance of Ta|Co and Pt|Co bilayers changes when reversing the polarity of the current or the sign of the magnetization. This unidirectional magnetoresistance scales linearly with current density and has opposite sign in Ta and Pt, which we associate with the modification of the interface scattering potential induced by the spin Hall effect in these materials. Our results suggest a route to control the resistance and detect magnetization switching in spintronic devices using a two-terminal geometry, which applies also to heterostructures including topological insulators.",1502.06898v2 2015-08-17,"Emergence of non-Fermi liquid behaviors in 5d perovskite SrIrO3 thin films: interplay between correlation, disorder, and spin-orbit coupling","We investigate the effects of compressive strain on the electrical resistivity of 5d iridium based perovskite SrIrO3 by depositing epitaxial films of thickness 35 nm on various substrates such as GdScO3 (110), DyScO3 (110), and SrTiO3 (001). Surprisingly, we find anomalous transport behaviors in the tempeature dependent resistivity, where the temperature exponent evolves continuously from 4/5 to 1 and to 3/2 with an increase of compressive strain. Furthermore, magnetoresistance always remains positive irrespective of resistivity upturns at low temperatures. These observations imply that the delicate interplay between correlation and disorder in the presence of strong spin-orbit coupling is responsible for the emergence of the non-Fermi liquid behaviors in 5d perovskite SrIrO3 thin films. We offer a theoretical framework for the interpretation of the experimental results.",1508.03944v1 2015-08-31,Scalable T^2 resistivity in a small single-component Fermi surface,"Scattering among electrons generates a distinct contribution to electrical resistivity that follows a quadratic temperature dependence. In strongly-correlated electron systems, the prefactor A of this T$^2$ resistivity scales with the magnitude of the electronic specific heat. Here, we show that one can change the magnitude of A by four orders of magnitude in metallic SrTiO3 by tuning the concentration of the carriers and consequently, the Fermi energy. The T$^2$ behavior persists in the single-band dilute limit despite the absence of two known mechanisms for T$^2$ behavior, distinct electron reservoirs and Umklapp processes. The results highlight the absence of a microscopic theory for momentum decay through electron-electron scattering in different Fermi liquids.",1508.07812v1 2015-08-31,In-Line-Test of Variability and Bit-Error-Rate of HfOx-Based Resistive Memory,"Spatial and temporal variability of HfOx-based resistive random access memory (RRAM) are investigated for manufacturing and product designs. Manufacturing variability is characterized at different levels including lots, wafers, and chips. Bit-error-rate (BER) is proposed as a holistic parameter for the write cycle resistance statistics. Using the electrical in-line-test cycle data, a method is developed to derive BERs as functions of the design margin, to provide guidance for technology evaluation and product design. The proposed BER calculation can also be used in the off-line bench test and build-in-self-test (BIST) for adaptive error correction and for the other types of random access memories.",1509.00070v1 2015-11-30,Solidification and loss of hydrostaticity in liquid media used for pressure measurements,"We carried out a study of the pressure dependence of the solidification temperature in nine pressure transmitting media that are liquid at ambient temperature, under pressures up to 2.3 GPa. These fluids are: 1:1 isopentane/n-pentane, 4:6 light mineral oil/n-pentane, 1:1 isoamyl alcohol/n-pentane, 4:1 methanol/ethanol, 1:1 FC72/FC84 (Fluorinert), Daphne 7373, isopentane, and Dow Corning PMX silicone oils 200 and 60,000 cst. We relied on the sensitivity of the electrical resistivity of Ba(Fe1-xRux)2As2 single crystals to the freezing of the pressure media, and cross-checked with corresponding anomalies observed in the resistance of the manganin coil that served as the ambient temperature resistive manometer. In addition to establishing the Temperature-Pressure line separating the liquid (hydrostatic) and frozen (non-hydrostatic) phases, these data permit rough estimates of the freezing pressure of these media at ambient temperature. This pressure establishes the extreme limit for the medium to be considered hydrostatic. For higher applied pressures the medium has to be treated as non-hydrostatic.",1512.00087v1 2015-12-18,The effect of quenching from different temperatures on Bi 0.88 Sb 0.12 alloy,"Structural, thermal, resistive and magnetic properties of melt quenched Bi 0.88 Sb 0.12 alloys are reported. The samples are heated at three different temperatures, followed by rapid quenching in liquid nitrogen. Large temperature difference between liquidus and solidus lines, led to microscopic in-homogeneity in the alloy. The effect of quenching from different temperatures in polycrystalline Bi 0.88 Sb 0.12 alloy has been studied. The parameters such as strain, unit cell volume, and resistivity are found to increase with temperature. Thermal variation of resistivity depicts non monotonic temperature dependence. The total negative susceptibility increases and band gap of semiconducting Bi 0.88 Sb 0.12 samples decreases with increasing temperature.",1512.05883v1 2015-12-18,Exchange Bias and Bistable Magneto-Resistance States in Amorphous TbFeCo thin Films,"Amorphous TbFeCo thin films sputter deposited at room temperature on thermally oxidized Si substrate are found to exhibit strong perpendicular magnetic anisotropy (PMA). Atom probe tomography (APT), scanning transmission electron microscopy (STEM), and energy dispersive spectroscopy (EDS) mapping have revealed two nanoscale amorphous phases with different Tb atomic percentages distributed within the amorphous film. Exchange bias accompanied by bistable magneto-resistance states has been uncovered near room temperature by magnetization and magneto-transport measurements. The exchange anisotropy originates from the exchange interaction between the ferrimagnetic and ferromagnetic components corresponding to the two amorphous phases. This study provides a platform for exchange bias and magneto-resistance switching using single-layer amorphous ferrimagnetic thin films that require no epitaxial growth.",1512.06103v1 2015-12-23,Topological Critical Point and Resistivity Anomaly in HfTe5,"There is a long-standing confusion concerning the physical origin of the anomalous resistivity peak in transition metal pentatelluride HfTe5. Several mechanisms, like the formation of charge density wave or polaron, have been proposed, but so far no conclusive evidence has been presented. In this work, we investigate the unusual temperature dependence of magneto-transport properties in HfTe5. We find that a three dimensional topological Dirac semimetal state emerges only at around Tp (at which the resistivity shows a pronounced peak), as manifested by a large negative magnetoresistance. This accidental Dirac semimetal state mediates the topological quantum phase transition between the two distinct weak and strong topological insulator phases in HfTe5. Our work not only provides the first evidence of a temperature-induced critical topological phase transition in HfTe5, but also gives a reasonable explanation on the long-lasting question.",1512.07360v1 2016-01-03,Detection of DC currents and resistance measurements in longitudinal spin Seebeck effect experiments on Pt/YIG and Pt/NFO,"In this work we investigated thin films of the ferrimagnetic insulators YIG and NFO capped with thin Pt layers in terms of the longitudinal spin Seebeck effect (LSSE). The electric response detected in the Pt layer under an out-of-plane temperature gradient can be interpreted as a pure spin current converted into a charge current via the inverse spin Hall effect. Typically, the transverse voltage is the quantity investigated in LSSE measurements (in the range of \mu V). Here, we present the directly detected DC current (in the range of nA) as an alternative quantity. Furthermore, we investigate the resistance of the Pt layer in the LSSE configuration. We found an influence of the test current on the resistance. The typical shape of the LSSE curve varies for increasing test currents.",1601.00304v1 2016-04-25,Anisotropic transport and optical spectroscopy study on antiferromagentic triangular lattice EuCd_2As_2: an interplay between magnetism and charge transport properties,"We present anisotropic transport and optical spectroscopy studies on EuCd_2As_2. The measurements reveal that EuCd_2As_2 is a low carrier density semimetal with moderate anisotropic resistivity ratio. The charge carriers experience very strong scattering from Eu magnetic moments, resulting in a Kondo-like increase of resistivity at low temperature. Below the antiferromagnetic transition temperature at $T_N$= 9.5 K, the resistivity drops sharply due to the reduced scattering from the ordered Eu moments. Nevertheless, the anisotropic ratio of $\rho_c/\rho_{ab}$ keeps increasing, suggesting that the antiferromagnetic coupling is along the c-axis. The optical spectroscopy measurement further reveals, besides an overdamped reflectance plasma edge at low energy, a strong coupling between phonon and electronic continuum. Our study suggests that EuCd_2As_2 is a promising candidate displaying intriguing interplay among charge, magnetism and the underlying crystal lattice.",1604.07114v2 2016-04-26,Multiband effects and the possible Dirac states in LaAgSb$_2$,"Here we report the possible signature of Dirac fermions in the magnetoresistance, Hall resistivity and magnetothermopower of LaAgSb$_2$. The opposite sign between Hall resistivity and Seebeck coefficient indicates the multiband effect. Electronic structure calculation reveals the existence of the linear bands and the parabolic bands crossing the Fermi level. The large linear magnetoresistance was attributed to the quantum limit of the possible Dirac fermions or the breakdown of weak-field magnetotransport at the charge density wave phase transition. Analysis of Hall resistivity using two-band model reveals that Dirac holes which dominate the electronic transport have much higher mobility and larger density than conventional electrons. Magnetic field suppresses the apparent Hall carrier density, and also induces the sign change of the Seebeck coefficient from negative to positive. These effects are possibly attributed to the magnetic field suppression of the density of states at the Fermi level originating from the quantum limit of the possible Dirac holes.",1604.07819v1 2016-04-27,Superconductivity at 7.8 K in the ternary LaRu2As2 compound,"Here we report the discovery of superconductivity in the ternary LaRu2As2 compound. The polycrystalline LaRu2As2 samples were synthesized by the conventional solid state reaction method. Powder X-ray diffraction analysis indicates that LaRu2As2 crystallizes in the ThCr2Si2-type crystal structure with the space group I4/mmm (No. 139), and the refined lattice parameters are a = 4.182(6) {\AA} and c = 10.590(3) {\AA}. The temperature dependent resistivity measurement shows a clear superconducting transition with the onset Tc (critical temperature) at 7.8 K, and zero resistivity happens at 6.8 K. The upper critical field at zero temperature m0Hc2(0) was estimated to be 1.6 T from the resistivity measurement. DC magnetic susceptibility measurement shows a bulk superconducting Meissner transition at 7.0 K, and the isothermal magnetization measurement indicates that LaRu2As2 is a type-II superconductor.",1604.07958v1 2016-06-02,First-principles calculation of the stabilities of lithium garnet compositions against hydration,"A series of density functional electronic structure calculations were carried out to better understand the crystallographic factors governing the stability of LinA3B2O12 lithium garnet phases against hydration. The reaction studied is H2O + LinA3B2O12 = LiOH + HnA3B2O12. Most of the compositions are stable against pure water; the main driving force for instability in the atmosphere is the reaction of lithium hydroxide with CO2 to make lithium carbonate. The calculated hydration resistance scales with the Pauling bond valence on the oxygen atom contributed by the coordinating A and B ions. In the unexchanged Li-garnets, this bond valence must be balanced by lithium, so there is also a good overall correlation of hydration stability with lithium stoichiometry (n): hydration resistance increases in the order Li8-garnet < Li7-garnet < Li6-garnet < Li5-garnet < Li3-garnet. Only Li3A3B2O12 garnets have proton exchange energies sufficiently positive to overcome the decomposition energy of lithium hydroxide into lithium carbonate + water; the n=3 garnets are predicted to be stable to hydration under atmospheric conditions, in agreement with observations (Galven et al. Chem. Mater. 2012 24, 3335-3345). At a given lithium ion stoichiometry, hydration resistance is greater for A, B ions having smaller ionic radii.",1606.01807v1 2016-06-07,The temperature dependence of FeRh's transport properties,"The finite-temperature transport properties of FeRh compounds are investigated by first-principles Density Functional Theory-based calculations. The focus is on the behavior of the longitudinal resistivity with rising temperature, which exhibits an abrupt decrease at the metamagnetic transition point, $T = T_m$ between ferro- and antiferromagnetic phases. A detailed electronic structure investigation for $T \geq 0$ K explains this feature and demonstrates the important role of (i) the difference of the electronic structure at the Fermi level between the two magnetically ordered states and (ii) the different degree of thermally induced magnetic disorder in the vicinity of $T_m$, giving different contributions to the resistivity. To support these conclusions, we also describe the temperature dependence of the spin-orbit induced anomalous Hall resistivity and Gilbert damping parameter. For the various response quantities considered the impact of thermal lattice vibrations and spin fluctuations on their temperature dependence is investigated in detail. Comparison with corresponding experimental data finds in general a very good agreement.",1606.02072v1 2016-06-21,Bad-Metal Relaxation Dynamics in a Fermi Lattice Gas,"We report the discovery of phenomena consistent with bad-metal relaxation dynamics in the metallic regime of an optical-lattice Hubbard model. The transport lifetime induced by inter-particle scattering for a mass current of atoms excited by stimulated Raman transitions is measured, and the corresponding analog of resistivity is inferred. By exploring a range of temperature, we demonstrate incompatibility with weak-scattering theory and a key characteristic of bad metals: anomalous resistivity scaling consistent with $T$-linear behavior. We also observe the onset of two behaviors---incoherent transport and the approach to the Mott-Ioffe-Regel limit---associated with bad metals. The interaction and temperature scaling of resistivity are verified to be consistent with dynamic mean-field theory (DMFT) predictions of a bad metal, which is associated with the reduction of quasiparticle weight by strong interactions.",1606.06669v5 2016-07-11,"The modification of the pore characteristics of activated carbon, for use in electrical double layer capacitors, through plasma processing","It was aimed to determine whether plasma processing could contribute to enhanced capacitance and energy density of activated carbon electrode based electrochemical capacitors, through the formation of additional surface charges. While an increase of up to 35% of the gravimetric capacitance, along with ~ 20% decrease in resistance, was obtained through optimal plasma processing, increased plasma exposure yielded a drastic reduction (/increase) in the capacitance (/resistance). It was also found that the capacitance and resistance modulation was a sensitive function of sample processing as well as electrochemical testing procedure. Considering the complexity of modeling realistic porous matrices, a metric to parameterize the reach of an electrolyte into the matrix has been posited.",1607.03201v1 2016-07-15,Chiral Phonons and Electrical Resistivity of Ferromagnetic Metals at Low Temperatures,"Ferromagnetism is an exciting phase of matter exhibiting strongly correlated electron behavior and a standard example of spontaneously broken rotational symmetry: below the Curie temperature, atomic magnets in an isotropic single-domain ferromagnetic metal align along a spontaneously chosen direction. The scattering of conduction electrons from thermal perturbations to this spin order, together with electron-electron collisions, mark the material electrical behavior at low temperatures, where the resistivity varies mostly quadratically with the temperature. Around liquid-helium temperatures however, an interesting phenomenon occurs, giving rise to an extra \emph{linear} contribution to the variation of the electrical resistivity with temperature, whose theoretical explanation has encountered problems for a long time. Here I introduce a spin-flip scattering mechanism of conduction electrons in ferromagnetic metals arising from their interaction with the internal magnetic induction and mediated by chiral modes of the crystal lattice vibrations carrying spin 1. This mechanism is able to explain the above anomaly and give a good account of the spin-lattice relaxation times of iron, cobalt and nickel at room temperatures.",1607.04585v2 2016-11-01,Boundary conditions and heat resistance at the moving solid--liquid interface,"Boundary conditions for the solid-liquid interface of the solidifying pure melt have been derived. In the derivation the model of Gibbs interface is used. The boundary conditions include both the state quantities of bulk phases are taken at the interface and the quantities characterizing interfacial surface such as the surface temperature and the surface heat flux. Introduction of the surface temperature as an independent variable allows us to describe the scattering energy at the interface. For the steady-state motion of the planar interface the expression for the temperature discontinuity across the phase boundary has been obtained. Effect of Kapitza resistance on the interface velocity is considered. It is shown that heat resistance leads to non-linearity in solidification kinetics, namely, in ""velocity-undercooling"" relationship. The conditions of the steady--state motion of the planar interface has been found.",1611.00160v1 2017-06-01,Edge transport in InAs and InAs/GaSb quantum wells,"We investigate low-temperature transport through single InAs quantum wells and broken-gap InAs/GaSb double quantum wells. Non-local measurements in the regime beyond bulk pinch-off confirm the presence of edge conduction in InAs quantum wells. The edge resistivity of 1-2 $\mathrm{k\Omega/\mu m}$ is of the same order of magnitude as edge resistivities measured in the InAs/GaSb double quantum well system. Measurements in tilted magnetic field suggests an anisotropy of the conducting regions at the edges with a larger extent in the plane of the sample than normal to it. Finger gate samples on both material systems shine light on the length dependence of the edge resistance with the intent to unravel the nature of edge conduction in InAs/GaSb coupled quantum wells.",1706.00320v1 2017-09-21,Zero-Field Quantum Critical Point in Ce$_{0.91}$Yb$_{0.09}$CoIn$_5$,"We present results of specific heat, electrical resistance, and magnetoresistivity measurements on single crystals of the heavy-fermion superconducting alloy Ce$_{0.91}$Yb$_{0.09}$CoIn$_5$. Non-Fermi liquid to Fermi liquid crossovers are clearly observed in the temperature dependence of the Sommerfeld coefficient $\gamma$ and resistivity data. Furthermore, we show that the Yb-doped sample with $x=0.09$ exhibits universality due to an underlying quantum phase transition without an applied magnetic field by utilizing the scaling analysis of $\gamma$. Fitting of the heat capacity and resistivity data based on existing theoretical models indicates that the zero-field quantum critical point is of antiferromagnetic origin. Finally, we found that at zero magnetic field the system undergoes a third-order phase transition at the temperature $T_{c3}\approx 7$ K.",1709.07161v3 2017-12-01,Titanium Contacts to Graphene: Process-Induced Variability in Electronic and Thermal Transport,"Contact Resistance (RC) is a major limiting factor in the performance of graphene devices. RC is sensitive to the quality of the interface and the composition of the contact, which are affected by the graphene transfer process and contact deposition conditions. In this work, a linear correlation is observed between the composition of Ti contacts, characterized by X-ray photoelectron spectroscopy, and the Ti/graphene (Gr) contact resistance measured by the transfer length method. We find that contact composition is tunable via deposition rate and base pressure. Reactor base pressure is found to effect the resultant contact resistance. The effect of contact deposition conditions on thermal transport measured by time-domain thermoreflectance is also reported and interfaces with higher oxide composition appear to result in a lower thermal boundary conductance. Possible origins of this thermal boundary conductance change with oxide composition are discussed.",1712.00331v1 2017-12-04,Particle-hole symmetry reveals failed superconductivity in the metallic phase of two-dimensional superconducting films,"Electrons confined to two dimensions display an unexpected diversity of behaviors as they are cooled to absolute zero. Noninteracting electrons are predicted to eventually ""localize"" into an insulating ground state, and it has long been supposed that electron correlations stabilize only one other phase: superconductivity. However, many two-dimensional (2D) superconducting materials have shown surprising evidence for metallic behavior, where the electrical resistivity saturates in the zero-temperature limit, the nature of this unexpected metallic state remains under intense scrutiny. We report electrical transport properties for two disordered 2D superconductors, indium oxide and tantalum nitride, and observe a magnetic field-tuned transition from a true superconductor to a metallic phase with saturated resistivity. This metallic phase is characterized by a vanishing Hall resistivity, suggesting that it retains particle-hole symmetry from the disrupted superconducting state.",1712.00947v1 2018-01-15,A study of electron and thermal transport in layered Titanium disulphide single crystals,"We present a detailed study of thermal and electrical transport behavior of single crystal Titanium disulphide flakes, which belongs to the two dimensional, transition metal dichalcogenide class of materials. In-plane Seebeck effect measurements revealed a typical metal-like linear temperature dependence in the range of 85 - 285 K. Electrical transport measurements with in-plane current geometry exhibited a nearly T^2 dependence of resistivity in the range of 10 - 300 K. However, transport measurements along the out-of-plane current geometry showed a transition in temperature dependence of resistivity from T^2 to T^5 beyond 200 K. Interestingly, Au ion-irradiated TiS2 samples showed a similar T 5 dependence of resistivity beyond 200 K, even in the current-in-plane geometry. Micro- Raman measurements were performed to study the phonon modes in both pristine and ion-irradiated TiS2 crystals.",1801.04677v1 2018-02-23,Possible charge-density-wave signatures in the anomalous resistivity of Li-intercalated multilayer MoS2,"We fabricate ion-gated field-effect transistors (iFET) on mechanically exfoliated multilayer MoS$_2$. We encapsulate the flake by Al$_2$O$_3$, leaving the device channel exposed at the edges only. A stable Li$^+$ intercalation in the MoS$_2$ lattice is induced by gating the samples with a Li-based polymeric electrolyte above $\sim$ 330 K and the doping state is fixed by quenching the device to $\sim$ 300 K. This intercalation process induces the emergence of anomalies in the temperature dependence of the sheet resistance and its first derivative, which are typically associated with structural/electronic/magnetic phase transitions. We suggest that these anomalies in the resistivity of MoS$_2$ can be naturally interpreted as the signature of a transition to a charge-density-wave phase induced by lithiation, in accordance with recent theoretical calculations.",1802.08449v2 2018-03-13,Are thermal fluctuations the sole reason for finite longitudinal resistance in quantum anomalous Hall experiments?,"In some recent experiments [A. J. Bestwick, et. al., Phys. Rev. Lett. 114, 187201 (2015), Cui-Zu Chang, et. al., Nat. Materials. 14, 473-477 (2015)] it has been shown that in observations of the quantum anomalous Hall (QAH) effect the longitudinal resistance $R_L$ increases as temperature $T$ increases, while Hall resistance $R_H$ loses its quantization with increase in $T$. This behavior was explained due to increased thermal fluctuations as $T$ increases. We show that similar effects arise in QAH samples with quasi-helical edge modes as disorder increases in presence of inelastic scattering or otherwise even at temperature $T=0$.",1803.04995v2 2018-03-21,Bad metallic transport in a modified Hubbard model,"Strongly correlated metals often display anomalous transport, including $T$-linear resistivity above the Mott-Ioffe-Regel limit. We introduce a tractable microscopic model for such bad metals, by supplementing the well-known Hubbard model --- with hopping $t$ and on-site repulsion $U$ --- with a `screened Coulomb' interaction between charge densities that decays exponentially with spatial separation. This interaction entirely lifts the extensive degeneracy in the spectrum of the $t=0$ Hubbard model, allowing us to fully characterize the small $t$ electric, thermal and thermoelectric transport in our strongly correlated model. Throughout the phase diagram we observe $T$-linear resistivity above the Mott-Ioffe-Regel limit, together with strong violation of the Weidemann-Franz law and a large thermopower that can undergo sign change. At intermediate temperatures $t \ll k_B T \lesssim U$, the approximate $T$-linear resistivity arises from a cancellation between the nontrivial temperature dependence of both diffusivities and thermodynamic susceptibilities, as observed in recent transport experiments on cold atomic gases.",1803.08054v3 2018-04-06,Energy-Quality Scaling in Analog Mesh Computers,"The recent push for post-Moore computer architectures has introduced a wide variety of application-specific accelerators. One particular accelerator, the resistance network analogue, has been well received due to its ability to efficiently solve partial differential equations by eliminating the iterative stages required by today's numerical solvers. However, in the ago of programmable integrated circuits, the static nature of the resistance network analogue, and other analog mesh computers like it, has relegated it to an academic curiosity. Recent developments in materials, such as the memristor, have made the resistance network analogue viable for inclusion in future heterogeneous computer architectures. However, selection of an appropriate sized mesh to be incorporated into a computer system requires that energy-quality trade-offs are made regarding the problem size and required resolution of the solution. This paper provides an in-depth study of the scaling of analog mesh computer hardware, from the perspective of energy per bit and required resolution, introduces a metric to aid in quantifying analog mesh computers with different parameters, and introduces a method of virtualization which enables an analog mesh computer of a fixed size to approximate the calculations of a larger-sized mesh.",1804.02389v2 2018-04-28,Nonequilibrium Mean-Field Theory of Resistive Phase Transitions,"We investigate the quantum mechanical origin of resistive phase transitions in solids driven by a constant electric field in the vicinity of a metal-insulator transition. We perform a nonequilibrium mean-field analysis of a driven-dissipative anti-ferromagnet, which we solve analytically for the most part. We find that the insulator-to-metal transition (IMT) and the metal-to-insulator transition (MIT) proceed by two distinct electronic mechanisms: Landau-Zener processes, and the destabilization of metallic state by Joule heating, respectively. However, we show that both regimes can be unified in a common effective thermal description, where the effective temperature $T_{\rm eff}$ depends on the state of the system. This explains recent experimental measurements in which the hot-electron temperature at the IMT was found to match the equilibrium transition temperature. Our analytic approach enables us to formulate testable predictions on the non-analytic behavior of $I$-$V$ relation near the insulator-to-metal transition. Building on these successes, we propose an effective Ginzburg-Landau theory which paves the way to incorporating spatial fluctuations, and to bringing the theory closer to a realistic description of the resistive switchings in correlated materials.",1804.10733v1 2018-09-24,Fusion Between Frozen-Wave-Type Beams and Airy-Type Pulses: Diffraction-Dispersion-Attenuation Resistant Vortex Pulses in Absorbing Media,"In this paper we perform a fusion between two important theoretical methodologies, one related to the Frozen Wave beams, which are non-diffracting beams whose longitudinal intensity pattern can be chosen a priori in an medium (absorbing or not), and the other related to the Airy-Type pulses, which are pulses resistant to dispersion effects in dispersive materials. As a result, a new method emerges, capable of providing vortex pulses resistant to three concomitant effects, i.e.: diffraction, dispersion and attenuation; while concurrently the spatial variation of the wave intensity along its axis of propagation can be engineered at will. The new approach can be seen as a generalization of the Localized Waves theory in the paraxial regime and the new pulses can have potential applications in different fields such as optics communications, nonlinear optics, micromanipulation, and so on.",1809.08740v1 2018-11-28,Investigation of effective thermoelectric properties of composite with interfacial resistance using micromechanics-based homogenisation,"We obtained the analytical expression for the effective thermoelectric properties and dimensionless figure of merit of a composite with interfacial electrical and thermal resistances using a micromechanics-based homogenisation. For the first time, we derived the Eshelby tensor for a spherical inclusion as a function of the interfacial resistances and obtained the solutions of the effective Seebeck coefficient and the electrical and thermal conductivities of a composite, which were validated against finite-element analysis (FEA). Our analytical predictions well match the effective properties obtained from FEA with an inclusion volume fraction up to 15%. Because the effective properties were derived with the assumption of a small temperature difference, we discuss a heuristic method for obtaining the effective properties in the case where a thermoelectric composite is subjected to a large temperature difference.",1811.11340v2 2019-05-13,Quantum Oscillations of Electrical Resistivity in an Insulator,"In metals, orbital motions of conduction electrons on the Fermi surface are quantized in magnetic fields, which is manifested by quantum oscillations in electrical resistivity. This Landau quantization is generally absent in insulators. Here we report a notable exception in an insulator, ytterbium dodecaboride (YbB12). Despite much larger than that of metals, the resistivity of YbB12 exhibits profound quantum oscillations. This unconventional oscillation is shown to arise from the insulating bulk, yet the temperature dependence of their amplitude follows the conventional Fermi liquid theory of metals. The large effective masses indicate the presence of Fermi surface consisting of strongly correlated electrons. Our result reveals a mysterious bipartite ground state of YbB12: it is both a charge insulator and a strongly correlated metal.",1905.05140v1 2019-09-27,Magnetoresistance effects in the metallic antiferromagnet Mn$_2$Au,"In antiferromagnetic spintronics, it is essential to separate the resistance modifications of purely magnetic origin from other effects generated by current pulses intended to switch the N\'eel vector. We investigate the magnetoresistance effects resulting from magnetic field induced reorientations of the staggered magnetization of epitaxial antiferromagnetic Mn2Au(001) thin films. The samples were exposed to 60 T magnetic field pulses along different crystallographic in-plane directions of Mn2Au(001), while their resistance was measured. For the staggered magnetization aligned via a spin-flop transition parallel to the easy [110]-direction, an ansiotropic magnetoresistance of -0.15 % was measured. In the case of a forced alignment of the staggered magnetization parallel to the hard [100]-direction, evidence for a larger anisotropic magnetoresistance effect was found. Furthermore, transient resistance reductions of about 1 % were observed, which we associate with the annihilation of antiferromagnetic domain walls by the magnetic field pulses.",1909.12606v3 2020-03-22,Monitoring of the formation of strontium molybdate intergrain tunneling barriers in strontium ferromolybdate,"This work is a contribution to the understanding of the electrical resistivity in strontium ferromolybdate (SFMO) ceramics. It demonstrates that an appropriate thermal treatment leads to the formation of dielectric SrMoO4 shells at the surface of SFMO nanograins. In samples without SrMoO4 shells, the sign of the temperature coefficient of resistance changes with increasing temperature from negative at very low temperature to positive at higher temperatures. Samples exhibiting a negative temperature coefficient contain SrMoO4 shells and demonstrate a behavior of the resistivity that can be described in terms of the fluctuation-induced tunneling model, and near room temperature the conductivity mechanism converts to a variable-range hopping one. The results of this work serve as a starting point for the understanding of the low-field magnetoresistance which is very promising for spintronic device application.",2003.09997v1 2014-08-15,Correlation between electrical and magnetic properties of phase separated manganites studied with a General Effective Medium model,"We have performed electrical resistivity and DC magnetization measurements as a function of temperature, on polycrystalline samples of phase separated LaPrCaMnO. We have used the General Effective Medium Theory to obtain theoretical resistivity vs. temperature curves corresponding to different fixed ferromagnetic volume fraction values, assuming that the sample is a mixture of typical metallic like and insulating manganites. By comparing this data with our experimental resistivity curves we have obtained the relative ferromagnetic volume fraction of our sample as a function of temperature. This result matches with the corresponding magnetization data in excellent agreement, showing that a mixed phase scenario is the key element to explain both the magnetic and transport properties in the present compound.",1408.3599v1 2014-08-28,Room temperature giant baroresistance and magnetoresistance and its tunability in Pd doped FeRh,"We report room temperature giant baro-resistance ($\approx$128\%) in $Fe_{49}(Rh_{0.93}Pd_{0.07})_{51}$. With the application of external pressure and magnetic field the temperature range of giant baro-resistance ($\approx$600\% at 5K and 19.9 kbar and 8 Tesla) and magnetoresistance ($\approx$-85\% at 5K and 8 tesla) can be tuned from 5 K to well above room temperature. As the AFM state is stabilized at room temperature under external pressure, it shows giant room temperature magnetoresistance ($\approx$-55\%) with magnetic field. Due to coupled magnetic and latticel changes, the isothermal change in room temperature resistivity with pressure (in the absence of applied magnetic field) as well as magnetic field (under various constant pressure) can be scaled together to a single curve when plotted as a function of X = T + 12.8*H - 7.2*P.",1408.6688v1 2017-01-18,Iron-based superconductivity extended to the novel silicide LaFeSiH,"We report the synthesis and characterization of the novel silicide LaFeSiH displaying superconductivity with onset at 11 K. We find that this pnictogen-free compound is isostructural to LaFeAsO, with a similar low-temperature tetragonal to orthorhombic distortion. Using density functional theory we show that this system is also a multiband metal in which the orthorhombic distortion is likely related to single-stripe antiferromagnetic order. Electrical resistivity and magnetic susceptibility measurements reveal that these features occur side-by-side with superconductivity, which is suppressed by external pressure.",1701.05010v3 2017-03-09,Oxygen migration during resistance switching and failure of hafnium oxide memristors,"While the recent establishment of the role of thermophoresis/diffusion-driven oxygen migration during resistance switching in metal oxide memristors provided critical insights required for memristor modeling, extended investigations of the role of oxygen migration during ageing and failure remain to be detailed. Such detailing will enable failure-tolerant design, which can lead to enhanced performance of memristor-based next-generation storage-class memory. Here we directly observed lateral oxygen migration using in-situ synchrotron x-ray absorption spectromicroscopy of HfOx memristors during initial resistance switching, wear over millions of switching cycles, and eventual failure, through which we determined potential physical causes of failure. Using this information, we reengineered devices to mitigate three failure mechanisms, and demonstrated an improvement in endurance of about three orders of magnitude.",1703.03106v1 2018-10-09,Electron scattering by short range defects and resistivity of graphene,"The electron scattering by the short-range defects in the monolayer graphene is considered in the framework of the flatland model. We analyze the effect of this scattering on the electronic resistivity of the monolayer graphene (direct problem) and develop a procedure for determination of the defect potential from resistivity data (inverse problem). We use an approximation of the short-range perturbation by the delta-shell potential that is reasonable since it suppresses irrelevant short wavelength excitations. Our theoretical results proved to be in a good agreement with experiment on suspended monolayer graphene. It means that our model correctly describes essential features of the physical problem under consideration. It gives possibility to consider the inverse problem, i.e. on the basis of our results for direct problem to develop a procedure for determination of parameters of the monolayer graphene sample using experimental measurements for it. Thus the obtained results give new important possibilities, which can be used in numerous applications.",1810.03897v1 2018-10-16,Studies of two-dimensional MoS2 on enhancing the electrical performance of ultrathin copper films,"Copper nanowires are widely used as on-chip interconnects due to superior conductivity. However, with aggressive Cu interconnect scaling, the diffusive surface scattering of electrons drastically increases the electrical resistivity. In this work, we studied the electrical performance of Cu thin films on different materials. By comparing the thickness dependence of Cu films resistivity on MoS2 and SiO2, we demonstrated that two-dimensional MoS2 can be used to enhance the electrical performance of ultrathin Cu films due to a partial specular surface scattering. By fitting the experimental data with the theoretical Fuchs Sondheimer model, we obtained the specularity parameter at the Cu MoS2 interface in the temperature range 2K to 300K. Furthermore, first principle calculations based on the density functional theory indicates that there are more localized states at the Cu amorphous SiO2 interface than the Cu MoS2 interface which is responsible for the higher resistivity in the Cu SiO2 heterostructure due to more severe electron scattering. Our results suggest that Cu MoS2 hybrid is a promising candidate structure for the future generations of CMOS interconnects.",1810.06772v1 2019-02-01,Graph Resistance and Learning from Pairwise Comparisons,"We consider the problem of learning the qualities of a collection of items by performing noisy comparisons among them. Following the standard paradigm, we assume there is a fixed ""comparison graph"" and every neighboring pair of items in this graph is compared $k$ times according to the Bradley-Terry-Luce model (where the probability than an item wins a comparison is proportional the item quality). We are interested in how the relative error in quality estimation scales with the comparison graph in the regime where $k$ is large. We prove that, after a known transition period, the relevant graph-theoretic quantity is the square root of the resistance of the comparison graph. Specifically, we provide an algorithm that is minimax optimal. The algorithm has a relative error decay that scales with the square root of the graph resistance, and provide a matching lower bound (up to log factors). The performance guarantee of our algorithm, both in terms of the graph and the skewness of the item quality distribution, outperforms earlier results.",1902.00141v2 2019-02-06,AlGaN /GaN superlattice based p-channel field effect transistor (pFET) with TMAH treatment,"To realize the full spectrum of advantages that the III-nitride materials system offers, the demonstration of p-channel III-nitride based devices is valuable. Authors report the first p-type field effect transistor (pFET) based on an AlGaN/GaN superlattice (SL), grown using MOCVD. Magnesium was used as the p-type dopant. A sheet resistance of 11.6 k{\Omega}/sq, and a contact resistance of 14.9{\Omega}.mm was determined using transmission line measurements (TLM) for a Mg doping of 1.5e19cm^-3 of Mg. Mobilities in the range of 7-10 cm\^2/Vs and a total sheet charge density in the range of 1e13-6e13 cm-2 were measured using room temperature Hall effect measurements. Without Tetramethylammonium hydroxide (TMAH) treatment, the fabricated pFETs had a maximum drain-source current (IDS) of 3mA/mm and an On-Resistance (RON) of 3.48 k{\Omega}.mm, and did not turn-off completely. With TMAH treatment during fabrication, a maximum IDS of 4.5mA/mm, RON of 2.2k{\Omega}.mm, and five orders of current modulation was demonstrated, which is the highest achieved for a p-type transistor based on (Al,Ga)N.",1902.02022v2 2019-02-26,Au-Ge alloys for wide-range low-temperature on-chip thermometry,"We present results of a Au-Ge alloy that is useful as a resistance-based thermometer from room temperature down to at least \SI{0.2}{\kelvin}. Over a wide range, the electrical resistivity of the alloy shows a logarithmic temperature dependence, which simultaneously retains the sensitivity required for practical thermometry while also maintaining a relatively modest and easily-measurable value of resistivity. We characterize the sensitivity of the alloy as a possible thermometer and show that it compares favorably to commercially-available temperature sensors. We experimentally identify that the characteristic logarithmic temperature dependence of the alloy stems from Kondo-like behavior induced by the specific heat treatment it undergoes.",1902.10111v2 2019-07-11,DC Electrical Degradation of YSZ: Voltage Controlled Electrical Metallization of A Fast Ion Conducting Insulator,"DC electrical degradation as a form of dielectric and resistance breakdown is a common phenomenon in thin-film devices including resistance-switching memory. To obtain design data and to probe the degradation mechanism, highly accelerated lifetime tests (HALT) are often conducted at higher temperatures with thicker samples. While the mechanism is well established in semiconducting oxides such as perovskite titanates, it is not in stabilized zirconia and other fast oxygen-ion conductors that have little electronic conductivity. Here we model the mechanism by an oxygen-driven, transport-limited, metal-insulator transition, which finds support in rich experimental observations - including in situ videos and variable temperature studies - of yttria-stabilized zirconia. They are contrasted with the findings in semiconducting titanates and resistance memory, and provide new insight into ceramic processing with extremely rapid heating and cooling such as flash sintering and melt processing.",1907.05479v2 2020-02-17,Transport mechanism in amorphous molybdenum silicide thin films,"Amorphous molybdenum silicide compounds have attracted significant interest for potential device applications, particularly in single-photon detector. In this work, the temperature-dependent resistance and magneto-resistance behaviors were measured to reveal the charge transport mechanism, which is of great importance for applications but is still insufficient. It is found that Mott variable hopping conductivity dominates the transport of sputtered amorphous molybdenum silicide thin films. Additionally, the observed magneto-resistance crossover from negative to positive is ascribed to the interference enhancement and the shrinkage of electron wave function, both of which vary the probability of hopping between localized sites.",2002.06884v3 2020-09-17,Restored strange metal phase through suppression of charge density waves in underdoped YBa$_2$Cu$_3$O$_{7-δ}$,"The normal state of optimally doped cuprates is dominated by the ""strange metal"" phase that shows a linear temperature ($T$) dependence of the resistivity persisting down to the lowest $T$. For underdoped cuprates this behavior is lost below the pseudogap temperature $T^*$, where Charge Density Waves (CDW) together with other intertwined local orders characterize the ground state. Here we show that the $T$-linear resistivity of highly strained, ultrathin and underdoped YBa$_2$Cu$_3$O$_{7-\delta}$ films is restored when the CDW amplitude, detected by Resonant Inelastic X-ray scattering, is suppressed. This observation points towards an intimate connection between the onset of CDW and the departure from $T$-linear resistivity in underdoped cuprates. Our results illustrate the potential of using strain control to manipulate the ground state of quantum materials.",2009.08398v3 2007-10-03,The effect of ozone oxidation on single-walled carbon nanotubes,"Exposing single-walled carbon nanotubes to room temperature UV-generated ozone leads to an irreversible increase in their electrical resistance. We demonstrate that the increased resistance is due to ozone oxidation on the sidewalls of the nanotubes rather than at the end caps. Raman and x-ray photoelectron spectroscopy show an increase in the defect density due to the oxidation of the nanotubes. Using ultraviolet photoelectron spectroscopy we show that these defects represent the removal of pi-conjugated electron states near the Fermi level, leading to the observed increase in electrical resistance. Oxidation of carbon nanotubes is an important first step in many chemical functionalization processes. Since the oxidation rate is controllable with short exposures, UV-generated ozone offers the potential for use as a low-thermal budget processing tool.",0710.0803v1 2012-01-13,Intermediate state switching dynamics in magnetic double layer nanopillars grown by molecular beam epitaxy,"We observe a stable intermediate resistance switching state in the current perpendicular to plane geometry for all Co/Cu/Co double layer nanopillar junctions grown by molecular beam epitaxy. This novel state has a resistance between the resistances of the parallel and antiparallel alignment of both Co-layer magnetizations. The state, which originates from an additional in-plane magnetic easy axis, can be reached by spin transfer torque switching or by an external magnetic field. In addition to spin torque-induced coherent small-angle spin wave modes we observe a broad microwave emission spectrum. The latter is attributed to incoherent magnetic excitations that lead to a switching between the intermediate state and the parallel or antiparallel alignment of both ferromagnetic layers. We conclude that the additional magnetic easy axis suppresses a stable trajectory of coherent large-angle precession, which is not observed in our samples.",1201.2752v1 2012-01-14,Length dependence of the resistance in graphite: Influence of ballistic transport,"Using a linear array of voltage electrodes with a separation of several micrometers on a $20 $nm thick and 30 $\mu$m long multigraphene sample we show that the measured resistance does not follow the usual length dependence according to Ohm's law. The deviations can be quantitatively explained taking into account Sharvin-Knudsen formula for ballistic transport. This allows us to obtain without free parameters the mean free path of the carriers in the sample at different temperatures. In agreement with recently reported values obtained with a different experimental method, we obtain that the carrier mean free path is of the order of $\sim 2 \mu$m with a mobility $\mu \sim 10^7 $cm$^{2}$V$^{-1}$s$^{-1}$. The results indicate that the usual Ohm's law is not adequate to calculate the absolute resistivity of mesoscopic graphite samples.",1201.3004v1 2012-01-14,Temperature dependence of the thermal boundary resistivity of glass-embedded metal nanoparticles,"The temperature dependence of the thermal boundary resistivity is investigated in glass-embedded Ag particles of radius 4.5 nm, in the temperature range from 300 to 70 K, using all-optical time-resolved nanocalorimetry. The present results provide a benchmark for theories aiming at explaining the thermal boundary resistivity at the interface between metal nanoparticles and their environment, a topic of great relevance when tailoring thermal energy delivery from nanoparticles as for applications in nanomedicine and thermal management at the nanoscale",1201.3034v1 2014-01-07,Images of edge current in InAs/GaSb quantum wells,"Quantum spin Hall devices with edges much longer than several microns do not display ballistic transport: that is, their measured conductances are much less than $e^2/h$ per edge. We imaged edge currents in InAs/GaSb quantum wells with long edges and determined an effective edge resistance. Surprisingly, although the effective edge resistance is much greater than $h/e^2$, it is independent of temperature up to 30 K within experimental resolution. Known candidate scattering mechanisms do not explain our observation of an effective edge resistance that is large yet temperature-independent.",1401.1531v2 2016-03-12,Spin Hall Effect and Origins of Nonlocal Resistance in Adatom-Decorated Graphene,"Recent experiments reporting unexpectedly large spin Hall effect (SHE) in graphene decorated with adatoms have raised a fierce controversy. We apply numerically exact Kubo and Landauer- Buttiker formulas to realistic models of gold-decorated disordered graphene (including adatom clustering) to obtain the spin Hall conductivity and spin Hall angle, as well as the nonlocal resistance as a quantity accessible to experiments. Large spin Hall angles of 0.1 are obtained at zero-temperature, but their dependence on adatom clustering differs from the predictions of semiclassical transport theories. Furthermore, we find multiple background contributions to the nonlocal resistance, some of which are unrelated to SHE or any other spin-dependent origin, as well as a strong suppression of SHE at room temperature. This motivates us to design a multiterminal graphene geometry which suppresses these background contributions and could, therefore, quantify the upper limit for spin current generation in two-dimensional materials.",1603.03870v3 2016-03-17,Electrical Writing of Magnetic and Resistive Multistates in CoFe Films Deposited onto Pb[Zr$_x$Ti$_{1-x}$]O$_3$,"Electric control of magnetic properties is an important challenge for modern magnetism and spintronic development. In particular, an ability to write magnetic state electrically would be highly beneficial. Among other methods, the use of electric field induced deformation of piezoelectric elements is a promising low-energy approach for magnetization control. We investigate the system of piezoelectric substrate Pb[Zr$_x$Ti$_{1-x}$]O$_3$ with CoFe overlayers, extending the known reversible bistable electro-magnetic coupling to surface and multistate operations, adding the initial state reset possibility. Increasing the CoFe thickness improves the magnetoresistive sensitivity, but at the expenses of decreasing the strain-mediated coupling, with optimum magnetic thin film thickness of the order of 100 nm. The simplest resistance strain gauge structure is realized and discussed as a multistate memory cell demonstrating both resistive memory (RRAM) and magnetoresistive memory (MRAM) functionalities in a single structure.",1603.05476v1 2018-08-26,Supercondutivity in SnSb with natural superlattice structure,"We report the results of electrical resistivity, magnetic and thermodynamic measurements on polycrystalline SnSb, whose structure consists of stacks of Sb bilayers and Sn4Sb3 septuple layers along the c-axis. The material is found to be a weakly coupled, fully gapped, type-II superconductor with a bulk Tc of 1.50 K, while showing a zero resistivity transition at a significantly higher temperature of 2.48 K. The Sommerfeld coefficient and upper critical field, obtained from specific heat measurements, are 2.29 mJ/mol K and 520 Oe, respectively. Compositional inhomogeneity and strain effect at the grain boundaries are proposed as possible origins for the difference in resistive and bulk superconducting transitions.In addition, a comparison with the rock-salt structure SnAs superconductor is presented. Our results provide the first clear evidence of bulk superconductivity in a natural superlattice derived from a topological semimetal.",1808.08500v2 2019-03-03,Scaling parameters in anomalous and nonlinear Hall effects depend on temperature,"In the study of the anomalous Hall effect, the scaling relations between the anomalous Hall and longitudinal resistivities play the central role. The scaling parameters by definition are fixed as the scaling variable (longitudinal resistivity) changes. Contrary to this paradigm, we unveil that the electron-phonon scattering can result in apparent temperature-dependence of scaling parameters when the longitudinal resistivity is tuned through temperature. An experimental approach is proposed to observe this hitherto unexpected temperature-dependence. We further show that this phenomenon also exists in the nonlinear Hall effect in nonmagnetic inversion-breaking materials and may help identify experimentally the presence of the side-jump contribution besides the Berry-curvature dipole.",1903.00810v5 2019-03-19,Composition dependence of magnetoresistance in Fe$_{1-x}$Ni$_{x}$ alloys,"Resistance of Fe$_{1-x}$Ni$_x$(x=0.1, 0.2, 0.3, 0.4, 0.5, 0.6, 0.7 and 0.9) has been measured using four probe method from 5K to 300K with and without a longitudinal magnetic field of 8T. The zero field resistivity of x=0.1 and 0.9 alloys, predominant contribution to resistivity above near room temperature is due to electron-phonon scattering, whereas for x=05 and 0.7 alloys electron-magnon scattering is dominant. Alloys with x=0.1 and 0.9 exhibit positive magnetoresistance(MR) from 5K to 300K. For x=0.5 and 0.7 alloys, magnetoresistance changes sign from positive to negative with increase in temperature. The temperature at which sign changes increase with Ni concentration in the alloy. The field dependent magnetoresistance is positive for x=0.1, 0.7 and 0.9 alloys whereas it is negative for x=0.5 alloy. MR follows linear behaviour with field for x=0.1 alloy. MR of all other alloys follow a second order polynomial in field.",1903.08230v3 2019-03-26,Controlled inter-state switching between quantized conductance states in resistive devices for multilevel memory,"A detailed understanding of quantization conductance (QC), their correlation with resistive switching phenomena and controlled manipulation of quantized states is crucial for realizing atomic-scale multilevel memory elements. Here, we demonstrate highly stable and reproducible quantized conductance states (QC-states) in Al/Niobium oxide/Pt resistive switching devices. Three levels of control over the QC-states, required for multilevel quantized state memories, like, switching ON to different quantized states, switching OFF from quantized states, and controlled inter-state switching among one QC states to another has been demonstrated by imposing limiting conditions of stop-voltage and current compliance. The well defined multiple QC-states along with a working principle for switching among various states show promise for implementation of multilevel memory devices.",1903.10688v1 2019-12-11,Current-induced fragmentation of antiferromagnetic domains,"Electrical and optical pulsing allow for manipulating the order parameter and magnetoresistance of antiferromagnets, opening novel prospects for digital and analog data storage in spintronic devices. Recent experiments in CuMnAs have demonstrated giant resistive switching signals in single-layer antiferromagnetic films together with analog switching and relaxation characteristics relevant for neuromorphic computing. Here we report simultaneous electrical pulsing and scanning NV magnetometry of antiferromagnetic domains in CuMnAs performed using a pump-probe scheme. We observe a nano-scale fragmentation of the antiferromagnetic domains, which is controlled by the current amplitude and independent on the current direction. The fragmented antiferromagnetic state conserves a memory of the pristine domain pattern, towards which it relaxes. Domain fragmentation coexists with permanent switching due to the reorientation of the antiferromagnetic moments. Our simultaneous imaging and resistance measurements show a correlation between the antiferromagnetic domain fragmentation and the largest resistive switching signals in CuMnAs.",1912.05287v1 2019-12-12,Aharonov-Bohm oscillations of four-probe resistance in topological quantum rings in silicene and bilayer graphene,"We consider observation of Aharonov-Bohm oscillations in clean systems based on the flow of topologically protected currents in silicene and bilayer graphene. The chiral channels in these materials are defined by the flips of the vertical electric field. The line of the flip confines chiral currents flowing along it in the direction determined by the valley. We present an electric field profile that forms a crossed ring to which four terminals can be attached, and find that the conductance matrix elements oscillate in the perpendicular magnetic field in spite of the absence of backscattering. We propose a four-probe resistance measurement setup, and demonstrate that the resistance oscillations have large visibility provided that the system is prepared in such a way that a direct transfer of the chiral carriers between the current probes is forbidden.",1912.05876v2 2021-01-13,Hinge Spin Polarization in Magnetic Topological Insulators Revealed by Resistance Switch,"We report on the possibility to detect hinge spin polarization in magnetic topological insulators by resistance measurements. By implementing a three-dimensional model of magnetic topological insulators into a multi-terminal device with ferromagnetic contacts near the top surface, local spin features of the chiral edge modes are unveiled. We find local spin polarization at the hinges that inverts sign between top and bottom surfaces. At the opposite edge, the topological state with inverted spin polarization propagates in the reverse direction. Large resistance switch between forward and backward propagating states is obtained, driven by the matching between the spin polarized hinges and the ferromagnetic contacts. This feature is general to the ferromagnetic, antiferromagnetic and canted-antiferromagnetic phases, and enables the design of spin-sensitive devices, with the possibility of reversing the hinge spin polarization of the currents.",2101.05293v2 2021-01-26,Demystifying strange metal and violation of Luttinger theorem in a doped Mott insulator,"Metallic states coined strange metal (SM), with robust linear-$T$ resistivity, have been widely observed in many quantum materials under strong electron correlation, ranging from high-$T_{c}$ cuprate superconductor, organic superconductor to twisted multilayer graphene and MoTe$_{2}$/WSe$_{2}$ superlattice. Despite decades of intensive studies, the mystery of strange metal still defies any sensible theoretical explanation and has been the key puzzle in modern condensed matter physics. Here, we solve a doped Mott insulator model, which unambiguously exhibits SM phenomena accompanied with quantum critical scaling in observables, e.g. resistivity, susceptibility and specific heat. Closer look at SM reveals the breakdown of Landau's Fermi liquid without any symmetry-breaking, i.e. the violation of Luttinger theorem. Examining electron's self-energy extracted from numerical simulation provides the explanation on the origin of linear-$T$ resistivity and suggests that the long-overlooked static fluctuations in literature play an essential role in non-Fermi liquid behaviors in correlated electron systems.",2101.10611v3 2012-06-15,A ferroelectric memristor,"Memristors are continuously tunable resistors that emulate synapses. Conceptualized in the 1970s, they traditionally operate by voltage-induced displacements of matter, but the mechanism remains controversial. Purely electronic memristors have recently emerged based on well-established physical phenomena with albeit modest resistance changes. Here we demonstrate that voltage-controlled domain configurations in ferroelectric tunnel barriers yield memristive behaviour with resistance variations exceeding two orders of magnitude and a 10 ns operation speed. Using models of ferroelectric-domain nucleation and growth we explain the quasi-continuous resistance variations and derive a simple analytical expression for the memristive effect. Our results suggest new opportunities for ferroelectrics as the hardware basis of future neuromorphic computational architectures.",1206.3397v1 2015-04-30,Study of the Negative Magneto-Resistance of Single Proton-Implanted Lithium-Doped ZnO Microwires,"The magneto-transport properties of single proton-implanted ZnO and of Li(7\%)-doped ZnO microwires have been studied. The as-grown microwires were highly insulating and not magnetic. After proton implantation the Li(7\%) doped ZnO microwires showed a non monotonous behavior of the negative magneto-resistance (MR) at temperature above 150 K. This is in contrast to the monotonous NMR observed below 50 K for proton-implanted ZnO. The observed difference in the transport properties of the wires is related to the amount of stable Zn vacancies created at the near surface region by the proton implantation and Li doping. The magnetic field dependence of the resistance might be explained by the formation of a magnetic/non magnetic heterostructure in the wire after proton implantation.",1504.08230v1 2015-07-29,Integration of a 2D Periodic Nanopattern Into Thin Film Polycrystalline Silicon Solar Cells by Nanoimprint Lithography,"The integration of two-dimensional (2D) periodic nanopattern defined by nanoimprint lithography and dry etching into aluminum induced crystallization (AIC) based polycrystalline silicon (Poly-Si) thin film solar cells is investigated experimentally. Compared to the unpatterned cell an increase of 6% in the light absorption has been achieved thanks to the nanopattern which, in turn, increased the short circuit current from 20.6 mA/cm2 to 23.8 mA/cm2. The efficiency, on the other hand, has limitedly increased from 6.4% to 6.7%. We show using the transfer length method (TLM) that the surface topography modification caused by the nanopattern has increased the sheet resistance of the antireflection coating (ARC) layer as well as the contact resistance between the ARC layer and the emitter front contacts. This, in turn, resulted in increased series resistance of the nanopatterned cell which has translated into a decreased fill factor, explaining the limited increase in efficiency.",1507.08341v1 2019-06-03,Observations of zero electrical resistance of Au-Ag thin films near room temperature,"Recent observations of superconducting like transition at 286 K in Ag and Ag nanostructures by Thapa et al. (arxiv: 1807.08572) have rekindled the hope for room temperature superconductivity under ambient conditions. We also investigated the electrical properties of Ag-Au nanostructure in the form of thin film grown on SiO2/Si substrate by DC sputtering and observed signature of zero resistance in the temperatures range of 243 K to 275 K. While the observed electrical resistance of samples shows intriguing and perplexing behavior under temperature cycling and external magnetic field; the large spatial inhomogeneity present in thin film hampers the reproducibility indicating the stability issues associated with superconducting like phase.",1906.00708v1 2019-06-24,Combination of informational storage and logical processing based on an all-oxide asymmetric multiferroic tunnel junction,"Multiferroic tunnel junctions (MFTJs) have already been proved to be promising candidates for application in spintronics devices. The coupling between tunnel magnetoresistance (TMR) and tunnel electroresistance (TER) in MFTJs can provide four distinct resistive states in a single memory cell. Here we show that in an all-oxide asymmetric MFTJ of La0.7Sr0.3MnO3 /PbZr0.2Ti0.8O3 /La0.7Te0.3MnO3 (LSMO/PZT/LTMO) with p-type and n-type electrodes, the intrinsic rectification is observed and can be modified by the ferroelectric polarization of PZT. Owing to the combined TMR, TER and diode effects, two different groups of four resistive states under opposite reading biases are performed. With two parallel asymmetric junctions and the appropriate series resistance, the coexistence of logic units and quaternary memory cells can be realized in the same array devices. The asymmetric MFTJ structure enables more possibilities for designing next generation of multi-states memory and logical devices with higher storage density, lower energy consumption and significantly increased integration level.",1906.09993v1 2019-10-04,Nonvolatile Multilevel States in Multiferroic Tunnel Junctions,"Manipulation of tunneling spin-polarized electrons via a ferroelectric interlayer sandwiched between two ferromagnetic electrodes, dubbed Multiferroic Tunnel Junctions (MFTJs), can be achieved not only by the magnetic alignments of two ferromagnets but also by the electric polarization of the ferroelectric interlayer, providing great opportunities for next-generation multi-state memory devices. Here we show that a La0.67Sr0.33MnO3 (LSMO)/PbZr0.2Ti0.8O3(PZT)/Co structured MFTJ device can exhibit multilevel resistance states in the presence of gradually reversed ferroelectric domains via tunneling electro-resistance and tunneling magnetoresistance, respectively. The nonvolatile ferroelectric control in the MFTJ can be attributed to separate contributions arising from two independent ferroelectric channels in the PZT interlayer with opposite polarization. Our study shows the dominant role of ""mixed"" ferroelectric states on achieving accumulative electrical modulation of multilevel resistance states in MFTJs, paving the way for multifunctional device applications.",1910.02002v1 2020-06-02,Ultra-fast Kinematic Vortices in Mesoscopic Superconductors: The Effect of the Self-Field,"Within the framework of the generalized time-dependent Ginzburg-Landau equations, we studied the influence of the magnetic self-field induced by the currents inside a superconducting sample driven by an applied transport current. The numerical simulations of the resistive state of the system show that neither material inhomogeneity nor a normal contact smaller than the sample width are required to produce an inhomogeneous current distribution inside the sample, which leads to the emergence of a kinematic vortex-antivortex pair (vortex street) solution. Further, we discuss the behaviors of the kinematic vortex velocity, the annihilation rates of the supercurrent, and the superconducting order parameters alongside the vortex street solution. We prove that these two latter points explain the characteristics of the resistive state of the system. They are the fundamental basis to describe the peak of the current-resistance characteristic curve and the location where the vortex-antivortex pair is formed.",2006.01335v1 2020-07-09,"Coupling-independent, Real-time Wireless Resistive Sensing through Nonlinear PT-symmetry","We report the realization of coupling-independent, robust wireless sensing of fully-passive resistive sensors. PT-symmetric operation obviates sweeping, permitting real-time, single-point sensing. Self-oscillation is achieved through a fast-settling nonlinearity whose voltage amplitude is proportional to the sensor's resistance. These advances markedly simplify the reader. A dual time-scale theoretical framework generalizes system analysis to arbitrary operating conditions and a correction strategy reduces errors due to detuning from PT-symmetric conditions by an order of magnitude.",2007.05077v4 2020-07-29,An electro-thermal computational study of conducting channels in dielectric thin films using self-consistent phase-field methodology: A view toward the physical origins of resistive switching,"A large number of experimental studies suggest two-terminal resistive switching devices made of a dielectric thin film sandwiched by a pair of electrodes exhibit reversible multi-state switching behaviors; however coherent understanding of physical and chemical origins of their electrical properties needs to be further pursued to improve and customize the performance. In this paper, phase-field methodology is used to study the formation and annihilation of conductive channels resulting in reversible resistive switching behaviors that can generally occur in any dielectric thin films. Our focus is on the dynamical evolution of domains made of electrical charges under the influence of spatially varying electric field and temperature resulting in distinctive changes in electrical conductance.",2007.15123v1 2020-08-24,Peierls-type metal-insulator transition in carbon nanostructures,"We report the observation of Peierls-type metal-insulator transition in carbon nanostructures formed by chemical vapor deposition inside the pore network of the ZSM-5 zeolite. The Raman spectrum of this nanocarbon@ZSM-5 indicates a clear signature of the radial breathing mode (RBM) for (3,0) carbon nanotubes that can constitute the carbon network segments. Electrical transport measurements on multiple few-micron-sized nanocarbon@ZSM-5 crystals showed metallic temperature of resistance dependence down to 30 K, at which point the resistance exhibited a sharp upturn that is accompanied by the opening of a quasigap at the Fermi level as indicated by the differential resistance measurements. Further Hall measurements have yielded both the sign of the charge carrier and its density. The latter demonstrated excellent consistency with the quasigap data. We employed first-principles calculations to verify that there can indeed be softening of the phonon modes in the (3,0) carbon nanotubes.",2008.10160v1 2020-10-22,Electrical and Thermal Transport Properties of the beta-Pyrochlore Oxide CsW2O6,"We report the electrical resistivity, thermoelectric power, and thermal conductivity of single-crystalline and sintered samples of the 5d pyrochlore oxide CsW2O6. The electrical resistivity of the single crystal is 3 mohm cm at 295 K and gradually increases with decreasing temperature above 215 K (Phase I). The thermoelectric power of the single-crystalline and sintered samples shows a constant value of approximately -60 uV K-1 in Phase I. These results reflect that the electron conduction by W 5d electrons in Phase I is incoherent and in the hopping regime, although a band gap does not open at the Fermi level. The thermal conductivity in Phase I of both samples is considerably low, which might be due to the rattling of Cs+ ions. In Phase II below 215 K, the electrical resistivity and the absolute value of thermoelectric power of both samples strongly increase with decreasing temperature, corresponding to a transition to a semiconducting state with a band gap open at the Fermi level, while the thermal conductivity in Phase II is smaller than that in Phase I.",2010.11404v1 2020-11-11,Elastic turbulence generates anomalous flow resistance in porous media,"Diverse processes rely on the viscous flow of polymer solutions through porous media. In many cases, the macroscopic flow resistance abruptly increases above a threshold flow rate in a porous medium---but not in bulk solution. The reason why has been a puzzle for over half a century. Here, by directly visualizing the flow in a transparent 3D porous medium, we demonstrate that this anomalous increase is due to the onset of an elastic instability. We establish that the energy dissipated by the unstable flow fluctuations, which vary across pores, generates the anomalous increase in flow resistance through the entire medium. Thus, by linking the pore-scale onset of unstable flow to macroscopic transport, our work provides generally-applicable guidelines for predicting and controlling polymer solution flows.",2011.06036v1 2021-02-08,Double magnetic phase transitions and magnetotransport anomalies in a new compound Gd$_\textbf{2}$AgSi$_\textbf{3}$,"Dc and ac-magnetic susceptibility ($\chi$), specific heat ($C_\mathrm{P}$), electrical resistivity ($\rho$) and magnetoresistance measurements performed on the new polycrystalline compound $\mathrm{Gd_2AgSi_3}$, crystallizing in the $\alpha$-$\mathrm{ThSi_2}$ tetragonal structure, are reported. Two magnetic phase transitions were observed in dc and ac susceptibility, specific heat, and resistivity measurements at temperatures $\mathrm{T_{N_1}} = 11$ K and $\rm{T_{N_2}} = 20$ K, despite a single site occupied by Gd atom, which is an indication of the complex magnetic behavior. $\mathrm{Gd_2AgSi_3}$ turns out to be one of the rare Gd compound in which a minimum is observed in the temperature dependence of resistivity in the paramagnetic state and also negative magnetoresistance over a wide temperature range (above $\rm{T_{N_2}}$), mimicking the behavior of exotic $\mathrm{Gd_2PdSi_3}$, in this ternary family. The isothermal magnetic entropy and adiabatic temperature changes reach a value of 9.5 J/kg-K and 7.5 K respectively for the field change of 9 T.",2102.04096v2 2021-04-23,Ab initio inspection of thermophysical experiments for zirconium near melting,"We present quantum molecular dynamics calculations of thermophysical properties of solid and liquid zirconium in the vicinity of melting. An overview of available experimental data is also presented. We focus on the analysis of thermal expansion, molar enthalpy, resistivity and normal spectral emissivity of solid and liquid Zr. Possible reasons of discrepancies between the first-principle simulations and experiments are discussed. Our calculations reveal a significant volume change on melting in agreement with electrostatic levitation experiments. Meanwhile, we confirm a low value of enthalpy of fusion obtained in some pulse-heating experiments. Electrical resistivity of solid and liquid Zr is systematically underestimated in our simulations, however the slope of resistivity temperature dependencies agrees with experiment. Our calculations predict almost constant normal spectral emissivity in liquid Zr.",2104.11521v2 2021-06-16,Statistical Analysis of Contacts to Synthetic Monolayer MoS2,"Two-dimensional (2D) semiconductors are promising candidates for scaled transistors because they are immune to mobility degradation at the monolayer limit. However, sub-10 nm scaling of 2D semiconductors, such as MoS2, is limited by the contact resistance. In this work, we show for the first time a statistical study of Au contacts to chemical vapor deposited monolayer MoS2 using transmission line model (TLM) structures, before and after dielectric encapsulation. We report contact resistance values as low as 330 ohm-um, which is the lowest value reported to date. We further study the effect of Al2O3 encapsulation on variability in contact resistance and other device metrics. Finally, we note some deviations in the TLM model for short-channel devices in the back-gated configuration and discuss possible modifications to improve the model accuracy.",2106.08673v3 2021-06-19,Dopant Precursor Adsorption into Single-Dimer Windows: Towards Guided Self-Assembly of Dopant Arrays on Si(100),"Atomically precise dopant arrays in Si are being pursued for solid-state quantum computing applications. We propose a guided self-assembly process to produce atomically precise arrays of single dopant atoms in lieu of lithographic patterning. We leverage the self-assembled c(4x2) structure formed on Br- and I-Si(100) and investigate molecular precursor adsorption into the generated array of single-dimer window (SDW) adsorption sites with density functional theory (DFT). The adsorption of several technologically relevant dopant precursors (PH$_3$, BCl$_3$, AlCl$_3$, GaCl$_3$) into SDWs formed with various resists (H, Cl, Br, I) are explored to identify the effects of steric interactions. PH$_3$ adsorbed without barrier on all resists studied, while BCl$_3$ exhibited the largest adsorption barrier, 0.34 eV, with an I resist. Dense arrays of AlCl$_3$ were found to form within experimentally realizable conditions demonstrating the potential for the proposed use of guided self-assembly for atomically precise fabrication of dopant-based devices.",2106.10556v1 2021-07-07,Large Magneto-Electric Resistance in the Topological Dirac Semimetal alpha Sn,"The spin-momentum locking of surface states in topological quantum materials can produce a resistance that scales linearly with magnetic and electric fields. Such a bilinear magneto-electric resistance (BMER) effect offers a completely new approach for magnetic storage and magnetic field sensing applications. The effects demonstrated so far, however, are relatively weak or for low temperatures. Strong room-temperature BMER effects have now been found in topological Dirac semimetal alpha-Sn thin films. The epitaxial alpha-Sn films were grown by sputtering on silicon substrates. They showed BMER responses that are 10^6 times larger than previously reported at room temperature and also larger than that previously reported at low temperatures. These results represent a major advance toward realistic BMER applications. The data also made possible the first characterization of the three-dimensional, Fermi-level spin texture of topological surface states in alpha-Sn.",2107.03472v1 2021-10-21,Magnetic critical behavior and anomalous Hall effect in 2H-Co$_{0.22}$TaS$_{2}$ single crystals,"We report ferromagnetism in 2H-Co$_{0.22}$TaS$_2$ single crystals where Co atoms are intercalated in the van der Waals gap, and a systematic study of its magnetic critical behavior in the vicinity of $T_c \sim 28$ K. The obtained critical exponents $\beta$ = 0.43(2), $\gamma$ = 1.15(1), and $\delta = 3.54(1)$ fulfill the Widom scaling relation $\delta = 1+\gamma/\beta$ and follow the scaling equation. This indicates that the spin coupling in 2H-Co$_{0.22}$TaS$_2$ is of three-dimensional Hersenberg type coupled with long-range magnetic interaction, and that the exchange interaction decays with distance as $J(r)\approx r^{-4.69}$. 2H-Co$_{0.22}$TaS$_2$ exhibits a weak temperature-dependent metallic behavior in resistivity and negative values of thermopower with dominant electron-type carriers, in which obvious anomalies were observed below $T_c$ as well as the anomalous Hall effect (AHE). The linear scaling behavior between the modified anomalous Hall resistivity $\rho_{xy}/\mu_0H$ and longitudinal resistivity $\rho_{xx}^2M/\mu_0H$ implies that the origin of AHE in 2H-Co$_{0.22}$TaS$_2$ should be dominated by the extrinsic side-jump mechanism.",2110.11350v1 2022-01-21,"Anomalous metals: from ""failed superconductor"" to ""failed insulator""","Resistivity saturation is found on both superconducting and insulating sides of an ""avoided"" magnetic-field-tuned superconductor-to-insulator transition (H-SIT) in a two-dimensional In/InO$_x$ composite, where the anomalous metallic behaviors cut off conductivity or resistivity divergence in the zero-temperature limit. The granular morphology of the material implies a system of Josephson junctions (JJ) with a broad distribution of Josephson coupling E$_J$ and charging energy E$_C$ , with a H-SIT determined by the competition between E$_J$ and E$_C$ . By virtue of self-duality across the true H-SIT, we invoke macroscopic quantum tunneling effects to explain the temperature-independent resistance where the ""failed superconductor"" side is a consequence of phase fluctuations and the ""failed insulator"" side results from charge fluctuations. While true self-duality is lost in the avoided transition, its vestiges are argued to persist, owing to the incipient duality of the percolative nature of the dissipative path in the underlying random JJ system.",2201.08801v1 2022-03-12,Quantifying active and resistive stresses in adherent cells,"To understand cell migration, it is crucial to gain knowledge on how cells exert and integrate forces on/from their environment. A quantity of prime interest for biophysicists interested in cell movements modeling is the intracellular stresses. Up to now, three different methods have been proposed to calculate it, they are all in the regime of the thin plate approximation. Two are based on solving the mechanical equilibrium equation inside the cell material (Monolayer Stress Microscopy, and Bayesian Inference Stress Microscopy) and one is based on the continuity of displacement at the cell/substrate interface (Intracellular Stress Microscopy). We show here using 3D FEM modeling that these techniques do not calculate the same quantities (as was previously assumed), the first techniques calculate the sum of the active and resistive stresses within the cell, whereas the last one only calculate the resistive component. Combining these techniques should in principle permit to get access to the active stress alone.",2203.06475v2 2022-03-23,Quantum oscillations and weak anisotropic resistivity in the chiral Fermion semimetal PdGa,"We perform a detailed analysis of the magnetotransport and de Haas-van Alphen (dHvA) oscillations in crystal PdGa which is predicted to be a typical chiral Fermion semimetal from CoSi family holding a large Chern number. The unsaturated quadratic magnetoresistance (MR) and nonlinear Hall resistivity indicate that PdGa is a multi-band system without electron-hole compensation. Angle-dependent resistivity in PdGa shows weak anisotropy with twofold or threefold symmetry when the magnetic field rotates within the (1$\bar{1}$0) or (111) plane perpendicular to the current. Nine or three frequencies are extracted after the fast Fourier-transform analysis (FFT) of the dHvA oscillations with B//[001] or B//[011], respectively, which is confirmed to be consistent with the Fermi surfaces (FSs) obtained from first-principles calculations with spin-orbit coupling (SOC) considered.",2203.12772v1 2022-05-04,Percolative Superconductivity in Electron-Doped Sr$_{1-x}$Eu$_{x}$CuO$_{2+y}$ Films,"Electron-doped infinite-layer Sr$_{1-x}$Eu$_{x}$CuO$_{2+y}$ films over a wide doping range have been prepared epitaxially on SrTiO$_3$(001) using reactive molecular beam epitaxy. In-plane transport measurements of the single crystalline samples reveal a dome-shaped nodeless superconducting phase centered at $x$ $\sim$ 0.15, a Fermi-liquid behavior and pronounced upturn in low temperature resistivity. We show that the resistivity upturn follows square-root temperature dependence, suggesting the emergence of superconductivity via a three-dimensional percolation process. The percolative superconductivity is corroborated spectroscopically by imaging the electronic phase separation between superconducting and metallic phases with low-temperature scanning tunneling microscopy. Furthermore, we visualize interstitial and apical oxygen anions that rapidly increase in number as $x>$ 0.12, and elucidate their impacts on the superconductivity and normal-state resistivity.",2205.01844v1 2022-05-10,Effect of substrate temperature on the optoelectronic properties of DC magnetron sputtered copper oxide films,"Copper oxide thin films are deposited on quartz substrates by DC magnetron sputtering and the effect of deposition temperature on their optoelectronic properties is examined in detail. Scanning Electron Microscopy (SEM), X-ray diffraction (XRD) analysis, Raman spectroscopy, UV-Vis spectroscopy, and four-probe sheet resistance measurements are used to characterize the surface morphology, structural, optical, and electrical properties respectively. Deposition is carried out at room temperature and between 200 and 300 {\deg}C. XRD analysis indicates that the oxide formed is primarily Cu$_2$O and the absorption spectra show the films have a critical absorption edge at around 300 nm. The sheet resistance gradually decreases with increase in deposition temperature thereby increasing the conductivity of these thin films. Also observed is the increase in band gap from 2.20 eV for room temperature deposition to 2.35 eV at 300 {\deg}C. The optical band gap and the variation of sheet resistance with temperature shows that the microstructure plays a vital role in their behavior. These transformation characteristics are of huge technological importance having variety of applications including transparent solar cell fabrication.",2205.05615v1 2022-08-10,Spin-carrier coupling induced ferromagnetism and giant resistivity peak in EuCd$_2$P$_2$,"EuCd$_2$P$_2$ is notable for its unconventional transport: upon cooling the metallic resistivity changes slope and begins to increase, ultimately 100-fold, before returning to its metallic value. Surprisingly, this giant peak occurs at 18K, well above the N\'{e}el temperature ($T_N$) of 11.5K. Using a suite of sensitive probes of magnetism, including resonant x-ray scattering and magneto-optical polarimetry, we have discovered that ferromagnetic order onsets above $T_N$ in the temperature range of the resistivity peak. The observation of inverted hysteresis in this regime shows that ferromagnetism is promoted by coupling of localized spins and itinerant carriers. The resulting carrier localization is confirmed by optical conductivity measurements.",2208.05499v1 2022-10-04,Time-domain impedance method for transient photovoltage analysis,"In this work, we approximate the surface photovoltage (SPV) transients in nm-sized ZnO films by the equivalent RC circuit model. The SPV rises in time in time for about 90 mcs after the exciting light pulse at 275 nm is off at different pulse widths ranging from 1.2 to 12 mcs. The key to this observation is a considerable amount of defects in the films, which form a trap capacitance in the equivalent circuit. The photogeneration of nonequilibrium electrons and holes near the film surface is described by charging of a capacitance by the current source whereas the rate of their spatial separation is determined by a resistance. This resistance reflects an obstacle in the carrier movement while another capacitance determines the charge separation distance. The electron-hole recombination is account for a second resistance introduced into the equivalent circuit. The resulting modeled SPV transient allows to reproduce the observed experimental curve rather well.",2210.07928v1 2022-10-17,Multiscale modeling of resistive switching in gold nanogranular films,"Metallic nanogranular films display a complex dynamical response to a constant bias, showing up as atypical resistive switching mechanism which could be used to create electrical components for neuromorphic applications. To model such a phenomenon we use a multiscale approach blending together an ab initio treatment of the electric current at the nanoscale, a molecular dynamical approach dictating structural rearrangements, and a finite-element solution of the heat equation for heat propagation in the sample. We also consider structural changes due to electromigration which are modelled on the basis of experimental observations on similar systems. Within such an approach, we manage to describe some distinctive features of the resistive switching occurring in nanogranular film and provide a physical interpretation at the microscopic level.",2210.09379v1 2022-10-27,Green's Functions For Random Resistor Networks,"We analyze random resistor networks through a study of lattice Green's functions in arbitrary dimensions. We develop a systematic disorder perturbation expansion to describe the weak disorder regime of such a system. We use this formulation to compute ensemble averaged nodal voltages and bond currents in a hierarchical fashion. We verify the validity of this expansion with direct numerical simulations of a square lattice with resistances at each bond exponentially distributed. Additionally, we construct a formalism to recursively obtain the exact Green's functions for finitely many disordered bonds. We provide explicit expressions for lattices with up to four disordered bonds, which can be used to predict nodal voltage distributions for arbitrarily large disorder strengths. Finally, we introduce a novel order parameter that measures the overlap between the bond current and the optimal path (the path of least resistance), for a given resistance configuration, which helps to characterize the weak and strong disorder regimes of the system.",2210.15562v3 2022-12-19,"Anisotropic resistance with a 90-degree twist in a ferromagnetic Weyl semimetal, Co2MnGa","Co$_2$MnGa is a ferromagnetic semimetal with Weyl nodal lines identified by ARPES. We studied electrical transport in thin Co$_2$MnGa lamellae (10 $\times$ 10 $\times$ 0.4-5 microns) cut from single-crystals using a focused ion beam. These crystals exhibit an unexpected and highly unusual planar resistance anisotropy ($\sim$10 times) with principal axes that rotate by 90 degrees between the upper and lower faces. Using symmetry arguments and simulations, we find that the observed resistance anisotropy resembles that of an isotropic conductor with anisotropic surface states that are impeded from hybridization with bulk states. The origin of these states awaits further experiments that can correlate the surface bands with the observed 90$^\circ$-twist geometry.",2212.09738v1 2022-12-29,Stateful Logic using Phase Change Memory,"Stateful logic is a digital processing-in-memory technique that could address von Neumann memory bottleneck challenges while maintaining backward compatibility with standard von Neumann architectures. In stateful logic, memory cells are used to perform the logic operations without reading or moving any data outside the memory array. Stateful logic has been previously demonstrated using several resistive memory types, mostly by resistive RAM (RRAM). Here we present a new method to design stateful logic using a different resistive memory - phase change memory (PCM). We propose and experimentally demonstrate four logic gate types (NOR, IMPLY, OR, NIMP) using commonly used PCM materials. Our stateful logic circuits are different than previously proposed circuits due to the different switching mechanism and functionality of PCM compared to RRAM. Since the proposed stateful logic form a functionally complete set, these gates enable sequential execution of any logic function within the memory, paving the way to PCM-based digital processing-in-memory systems.",2212.14377v1 2023-03-15,Two-fold anisotropic superconducting state in topological superconductor Sn$_4$Au,"Here we report the anisotropic magnetotransport properties in the superconducting state of Sn$_4$Au single crystal. Sn$_4$Au single crystal is synthesized through an easy melt growth method. Superconducting properties are evidenced by resistivity vs. temperature and DC magnetization measurements. Isothermal magnetization measurements hint toward type-II superconductivity in Sn$_4$Au. In-plane and out-of-plane resistivity measurements show anisotropic behavior of the upper critical field at temperatures below superconducting transition (T$_c$ = 2.3 K). The observed anisotropy is more elucidated in resistivity measurements performed below Tc at different tilt angles. The anisotropy parameter is found to be 1.26. The observed results show the presence two-fold anisotropic superconducting state in Sn$_4$Au single crystal, which may be induced due to the layered structure of synthesized Sn$_4$Au single crystal.",2303.08520v1 2023-03-28,Effect of atomic anti-site disorder on the AMR in FeCo alloys,"In order to understand the anti-site disorder effect on the anisotropic magnetoresistance (AMR) effect in alloys, $\rm{Fe}_{50}Co_{50}$ alloys were studied in this work using the fully relativistic spin-polarized screened (KKR) method. The anti-site effect was modeled by interchanging Fe and Co atoms and treated by the coherent potential approximation (CPA). We find that the anti-site disorder broadens the spectral function and decreases the conductivity. Our work emphasizes that the absolute variations of resistivity under magnetic moment rotation are less affected by atomic disorders. The annealing procedure improves the AMR by reduction of the total resistivity. At the same time, we also find that the fourth-order term in the angular dependent resistivity becomes weaker when the disorder increases, resulting from increased scattering of the states around the band-crossing.",2303.15726v1 2023-03-28,Superconductivity in boron-doped carbon nanotube networks,"By using the five Angstrom diameter pores of calcined zeolite as the template, we have fabricated boron doped carbon nanotube networks via the chemical vapor deposition method. Raman data indicate the network to comprise segments of interconnected carbon nano tubes. Transport measurements showed a superconducting transition initiating at 40K, with a sharp downturn around 20K to a low resistance state at 2K, accompanied by a low resistance plateau in the current voltage characteristic, fluctuating around zero resistance. Magnetic measurements exhibited the Meissner effect characteristic of thin superconducting wire networks in which the superconducting wire radius is much smaller than the London penetration length. At low magnetic field, the negative diamagnetic susceptibility was observed to persist beyond 200K. The transport and magnetic data are reconciled on the basis of a physical model based on weak links comprising short, one-dimensional superconducting nano tubes, that govern the global transport behavior.",2303.15980v1 2023-04-12,Measuring a Soft Resistive Strain Sensor Array by Solving the Resistor Network Inverse Problem,"Soft robotics is applicable to a variety of domains due to the adaptability offered by the soft and compliant materials. To develop future intelligent soft robots, soft sensors that can capture deformation with nearly infinite degree-of-freedom are necessary. Soft sensor networks can address this problem, however, measuring all sensor values throughout the body requires excessive wiring and complex fabrication that may hinder robot performance. We circumvent these challenges by developing a non-invasive measurement technique, which is based on an algorithm that solves the inverse problem of resistor network, and implement this algorithm on a soft resistive, strain sensor network. Our algorithm works by iteratively computing the resistor values based on the applied boundary voltage and current responses, and we analyze the reconstruction error of the algorithm as a function of network size and measurement error. We further develop electronics setup to implement our algorithm on a stretchable resistive strain sensor network made of soft conductive silicone, and show the response of the measured network to different deformation modes. Our work opens a new path to address the challenge of measuring many sensor values in soft sensors, and could be applied to soft robotic sensor systems.",2304.05828v1 2023-05-22,Ion-selective scattering studied by the variable-energy electron irradiation of Ba$_{0.2}$K$_{0.8}$Fe$_2$As$_2$ superconductor,"Low-temperature variable-energy electron irradiation was used to induce non-magnetic disorder in a single crystal of hole-doped iron-based superconductor, Ba$_{1-x}$K$_x$Fe$_2$As$_2$, $x=$0.80. To avoid systematic errors, the beam energy was adjusted non-consequently for five values between 1.0 and 2.5 MeV, whence sample resistance was measured in-situ at 22 K. For all energies, the resistivity raises linearly with the irradiation fluence suggesting the creation of uncorrelated dilute point-like disorder (confirmed by simulations). The rate of the resistivity increase peaks at energies below 1.5 MeV. Comparison with calculated partial cross-sections points to the predominant creation of defects in the iron sublattice. Simultaneously, superconducting $T_c$, measured separately between the irradiation runs, is monotonically suppressed as expected since it depends on the total scattering rate, hence total cross-section, which is a monotonically increasing function of energy. Our work confirms experimentally an often-made assumption of the dominant role of the iron sub-lattice in iron-based superconductors.",2305.13217v1 2023-06-05,Multilayer GZ/YSZ Thermal Barrier Coating from Suspension and Solution Precursor Plasma Spray,"Gas turbines rely on thermal barrier coating (TBC) to thermally insulate the nickel-based superalloys underneath during operation; however, current TBCs, yttria stabilised zirconia (YSZ), limit the operating temperature and hence efficiency. At an operating temperature above 1200{\deg}C, YSZ is susceptible to failure due to phase instabilities and CMAS (Calcia-Magnesia-Alumina-Silica) attack. Gadolinium zirconates (GZ) could overcome the drawback of YSZ, complementing each other with the multi-layer approach. This study introduces a novel approach utilising axial suspension plasma spray (ASPS) and axial solution precursor plasma spray (ASPPS) to produce a double-layer and a triple-layer TBCs with improved CMAS resistance. The former comprised suspension plasma sprayed GZ and YSZ layers while the latter had an additional dense layer deposited through a solution precursor to minimise the columnar gaps that pre-existed in the SPS GZ layer, thus resisting CMAS infiltration. Both coatings performed similarly in furnace cycling test (FCT) and burner rig testing (BRT). In the CMAS test, triple-layer coating showed better CMAS resistivity, as evidenced by the limited CMAS infiltration observed on the surface.",2306.02720v1 2024-01-31,Effect of severe plastic deformation realized by rotary swaging on the mechanical properties and corrosion resistance of near-a-titanium alloy Ti-2.5Al-2.6Zr,"The research aims to analyze the impact that severe plastic deformation arising during Rotary Swaging has on mechanical properties and corrosion resistance of a near-a-titanium alloy Ti-2.5Al-2.6Zr (Russian industrial name PT7M). The nature of corrosion decay in fine-grained alloys caused by hot salt corrosion is known to vary from pit corrosion to intercrystalline corrosion at the onset of recrystallization processes. Resistance to hot salt corrosion in a fine-grained titanium alloy Ti-2.5Al-2.6Zr is shown to depend on the structural-phase state of grain boundaries that varies during their migration as a result of covering corrosive doping elements (aluminum, zirconium) distributed in the crystal lattice of a titanium alloy.",2401.17672v1 2024-03-17,Observation of diamagnetic strange-metal phase in sulfur-copper codoped lead apatite,"By codoping sulfur and copper into lead apatite, the crystal grains are directionally stacked and the room-temperature resistivity is reduced from insulating to $2\times10^{-5}~\Omega\cdot$m. The resistance-temperature curve exhibits a nearly linear relationship at low temperature suggesting the presence of strange-metal phase, and a second-order phase transition is then observed at around 230~K during cooling the samples. A possible Meissner effect is present in dc magnetic measurements. Further hydrothermal lead-free synthesis results in smaller resistance and stronger diamagnetism, demonstrating the essential component might be sulfur-substituted copper apatite and the alkalis matter as well. A clear pathway towards superconductivity in this material is subsequently benchmarked.",2403.11126v3 2024-04-09,Transport resistance strikes back: unveiling its impact on fill factor losses in organic solar cells,"The fill factor ($FF$) is a critical parameter for solar cell efficiency, yet its analytical description is challenging due to the interplay between recombination and charge extraction processes. An often overlooked yet significant factor contributing to $FF$ losses, beyond recombination, is the influence of charge transport. In most state-of-the-art organic solar cells, the primary limitation of the $FF$ arises not from recombination but rather from low conductivity, highlighting the need for refined models to predict the $FF$ accurately. Here, we extend the analytical model for transport resistance to a more general case. Drawing from a large set of experimental current-voltage and light intensity-dependent open-circuit voltage data, we systematically incorporate crucial details previously omitted in the model. Consequently, we introduce a straightforward set of equations to predict the $FF$ of a solar cell, enabling the differentiation of losses attributed to recombination and transport resistance. Our study provides valuable insights into strategies for mitigating $FF$ losses based on the experimentally validated analytical model, guiding the development of more efficient solar cell designs and optimization strategies.",2404.06190v1 2024-05-09,Negative longitudinal resistance of monolayer graphene in the quantum Hall regime,"In the quantum Hall regime the charge current is carried by ideal one-dimensional edge channels where the backscattering is prohibited by topology. This results in the constant potential along the edge of the Hall bar leading to zero 4-terminal longitudinal resistance r_xx. Finite scattering between the counter-propagating edge states, when the topological protection is broken, commonly results in r_xx > 0. However, a local disorder, if allowing intersection of the edge states, can result in a counter-intuitive scenario when r_xx<0. In this work we report the observation and a systematic study of such unconventional negative longitudinal resistance seen in an encapsulated monolayer graphene Hall bar device measured in the quantum Hall regime. We supplement our findings with the numerical calculations which allow us to outline the conditions necessary for the appearance of negative r_xx and to exclude the macroscopic disorder (contamination bubble) as the main origin of it.",2405.05515v2 2012-08-01,Spin-fluctuations in Ti$_{60}$V$_{40}$ alloy and its influence on the superconductivity,"We report experimental studies of the temperature and magnetic field dependence of resistivity and dc magnetic susceptibility and the temperature dependence of zero field heat capacity in a Ti$_{0.6}$V$_{0.4}$ alloy. The temperature dependence of the normal state dc magnetic susceptibility in this Ti$_{0.6}$V$_{0.4}$ alloy shows T$^2$lnT behavior. The temperature dependence of resistivity follows a T$^2$ behaviour in the range 20-50 K. On the other hand, a term $T^3$ lnT is needed in the expression containing the electronic and lattice heat capacities to explain the temperature dependence of heat capacity at temperatures where $T^2$ dependence of resistivity is observed. Such temperature dependence of dc magnetic susceptibility, resistivity and heat capacity are indications of the presence of spin-fluctuations in the system. Further experimental evidence for the spin fluctuations is obtained in the form of a negative value of T$^5$ term in the temperature dependence of resistivity. The influence of spin-fluctuations on the superconducting properties of Ti$_{0.6}$V$_{0.4}$ is discussed in detail. We show from our analysis of resistivity and the susceptibility in normal and superconducting states that the spin fluctuations present in Ti$_{0.6}$V$_{0.4}$ alloy are itinerant in nature. There is some evidence of the existence of preformed Cooper-pairs in the temperature range well above the superconducting transition temperature. Our study indicates that the interesting correlations between spin-fluctuations and superconductivity may actually be quite widespread amongst the superconducting materials, and not necessarily be confined only to certain classes of exotic compounds.",1208.0181v3 2016-06-14,On the multiferroic skyrmion-host GaV4S8,"The lacunar spinel GaV4S8 exhibits orbital ordering at 44 K and shows a complex magnetic phase diagram below 12.7 K, which includes ferromagnetic and cycloidal spin order. At low but finite external magnetic fields, N\'eel-type skyrmions are formed in this material. Skyrmions are whirl-like spin vortices that have received great theoretical interest because of their non-trivial spin topology and that are also considered as basic entities for new data-storage technologies. Interestingly, we found that the orbitally ordered phase shows sizable ferroelectric polarization and that excess spin-driven polarizations appear in all magnetic phases, including the skyrmion-lattice phase. Hence, GaV4S8 shows simultaneous magnetic and polar order and belongs to the class of multiferroics, materials that attracted enormous attention in recent years. Here, we summarize the existing experimental information on the magnetic, electronic, and dielectric properties of GaV4S8. By performing detailed magnetic susceptibility, resistivity, specific heat, and dielectric experiments, we complement the low-temperature phase diagram. Specifically, we show that the low-temperature and low-field ground state of GaV4S8 seems to have a more complex spin configuration than purely collinear ferromagnetic spin order. In addition, at the structural Jahn-Teller transition the magnetic exchange interaction changes from antiferromagnetic to ferromagnetic. We also provide experimental evidence that the vanadium V4 clusters in GaV4S8 can be regarded as molecular units with spin 1/2. However, at high temperatures deviations in the susceptibility show up, indicating that either the magnetic moments of the vanadium atoms fluctuate independently or excited states of the V4 molecule become relevant.",1606.04511v1 2016-10-24,Self-aligned local electrolyte gating of 2D materials with nanoscale resolution,"In the effort to make 2D materials-based devices smaller, faster, and more efficient, it is important to control charge carrier at lengths approaching the nanometer scale. Traditional gating techniques based on capacitive coupling through a gate dielectric cannot generate strong and uniform electric fields at this scale due to divergence of the fields in dielectrics. This field divergence limits the gating strength, boundary sharpness, and pitch size of periodic structures, and restricts possible geometries of local gates (due to wire packaging), precluding certain device concepts, such as plasmonics and transformation optics based on metamaterials. Here we present a new gating concept based on a dielectric-free self-aligned electrolyte technique that allows spatially modulating charges with nanometer resolution. We employ a combination of a solid-polymer electrolyte gate and an ion-impenetrable e-beam-defined resist mask to locally create excess charges on top of the gated surface. Electrostatic simulations indicate high carrier density variations of $\Delta n =10^{14}\text{cm}^{-2}$ across a length of 10 nm at the mask boundaries on the surface of a 2D conductor, resulting in a sharp depletion region and a strong in-plane electric field of $6\times10^8 \text{Vm}^{-1}$ across the so-created junction. We apply this technique to the 2D material graphene to demonstrate the creation of tunable p-n junctions for optoelectronic applications. We also demonstrate the spatial versatility and self-aligned properties of this technique by introducing a novel graphene thermopile photodetector.",1610.07646v2 2020-09-22,Half-Metal Spin-Gapless Semiconductor Junctions as a Route to the Ideal Diode,"The ideal diode is a theoretical concept that completely conducts the electric current under forward bias without any loss and that behaves like a perfect insulator under reverse bias. However, real diodes have a junction barrier that electrons have to overcome and thus they have a threshold voltage $V_T$, which must be supplied to the diode to turn it on. This threshold voltage gives rise to power dissipation in the form of heat and hence is an undesirable feature. In this work, based on half-metallic magnets and spin-gapless semiconductors we propose a diode concept that does not have a junction barrier and the operation principle of which relies on the spin-dependent transport properties of the HMM and SGS materials. We show that the HMM and SGS materials form an Ohmic contact under any finite forward bias, while for a reverse bias the current is blocked due to spin-dependent filtering of the electrons. Thus, the HMM-SGS junctions act as a diode with zero threshold voltage $V_T$, and linear $I-V$ characteristics as well as an infinite on:off ratio at zero temperature. However, at finite temperatures, non-spin-flip thermally excited high-energy electrons as well as low-energy spin-flip excitations can give rise to a leakage current and thus reduce the on:off ratio under a reverse bias. Furthermore, a zero threshold voltage allows one to detect extremely weak signals and due to the Ohmic HMM-SGS contact, the proposed diode has a much higher current drive capability and low resistance, which is advantageous compared to conventional semiconductor diodes. We employ the NEGF method combined with DFT to demonstrate the linear $I-V$ characteristics of the proposed diode based on two-dimensional half-metallic Fe/MoS$_2$ and spin-gapless semiconducting VS$_2$ planar heterojunctions.",2009.10463v1 2020-11-22,"Quasi-two-dimensional heterostructures (K$M_{1-x}$Te)(LaTe$_{3}$) ($M$ = Mn, Zn) with charge density waves","Layered heterostructure materials with two different functional building blocks can teach us about emergent physical properties and phenomena arising from interactions between the layers. We report the intergrowth compounds KLa$M$$_{1-x}$Te$_{4}$ ($M$ = Mn, Zn; $x\approx$ 0.35) featuring two chemically distinct alternating layers [LaTe$_3$] and [K$M$$_{1-x}$Te]. Their crystal structures are incommensurate, determined by single X-ray diffraction for the Mn compound and transmission electron microscope (TEM) study for the Zn compound. KLaMn$_{1-x}$Te$_{4}$ crystallizes in the orthorhombic superspace group $Pmnm$(01/2${\gamma}$)$s$00 with lattice parameters $a$ = 4.4815(3) {\AA}, $b$ = 21.6649(16) {\AA} and $c$ = 4.5220(3) {\AA}. It exhibits charge density wave (CDW) order at room temperature with a modulation wave vector $\mathbf{q}$ = 1/2$\mathbf{b}$* + 0.3478$\mathbf{c}$* originating from electronic instability of Te-square nets in [LaTe$_{3}$] layers. The Mn analog exhibits a cluster spin glass behavior with spin freezing temperature $T_{\mathrm{f}}$ $\approx$ 5 K attributed to disordered Mn vacancies and competing magnetic interactions in the [Mn$_{1-x}$Te] layers. The Zn analog also has charge density wave order at room temperature with a similar $\mathbf{q}$-vector having the $\mathbf{c}$* component ~ 0.346 confirmed by selected-area electron diffraction (SAED). Electron transfer from [K$M_{1-x}$Te] to [LaTe$_{3}$] layers exists in KLa$M_{1-x}$Te$_{4}$, leading to an enhanced electronic specific heat coefficient. The resistivities of KLa$M_{1-x}$Te$_{4}$ ($M$ = Mn, Zn) exhibit metallic behavior at high temperatures and an upturn at low temperatures, suggesting partial localization of carriers in the [LaTe$_{3}$] layers with some degree of disorder associated with the $M$ atom vacancies in the [$M_{1-x}$Te] layers.",2011.11068v2 2021-06-09,Fracture Mechanics-Based Quantitative Matching of Forensic Evidence Fragments,"Fractured metal fragments with rough and irregular surfaces are often found at crime scenes. Current forensic practice visually inspects the complex jagged trajectory of fractured surfaces to recognize a ``match'' using comparative microscopy and physical pattern analysis. We developed a novel computational framework, utilizing the basic concepts of fracture mechanics and statistical analysis to provide quantitative match analysis for match probability and error rates. The framework employs the statistics of fracture surfaces to become non-self-affine with unique roughness characteristics at relevant microscopic length scale, dictated by the intrinsic material resistance to fracture and its microstructure. At such a scale, which was found to be greater than two grain-size or micro-feature-size, we establish that the material intrinsic properties, microstructure, and exposure history to external forces on an evidence fragment have the premise of uniqueness, which quantitatively describes the microscopic features on the fracture surface for forensic comparisons. The methodology utilizes 3D spectral analysis of overlapping topological images of the fracture surface and classifies specimens with very high accuracy using statistical learning. Cross correlations of image-pairs in two frequency ranges are used to develop matrix variate statistical models for the distributions among matching and non-matching pairs of images, and provides a decision rule for identifying matches and determining error rates. A set of thirty eight different fracture surfaces of steel articles were correctly classified. The framework lays the foundations for forensic applications with quantitative statistical comparison across a broad range of fractured materials with diverse textures and mechanical properties.",2106.04809v1 2021-06-16,Role of surface termination in the metal-insulator transition of V$_2$O$_3$(0001) ultrathin films,"Surface termination is known to play an important role in determining the physical properties of materials. It is crucial to know how surface termination affects the metal-insulator transition (MIT) of V$_2$O$_3$ films for both fundamental understanding and its applications. By changing growth parameters, we achieved a variety of surface terminations in V$_2$O$_3$ films that are characterized by low energy electron diffraction (LEED) and photoemission spectroscopy techniques. Depending upon the terminations, our results show MIT can be partially or fully suppressed near the surface region due to the different filling of the electrons at the surface and sub-surface layers and change of screening length compared to the bulk. Across MIT, a strong redistribution of spectral weight and its transfer from high-to-low binding energy regime is observed in a wide-energy-scale. Our results show total spectral weight in the low-energy regime is not conserved across MIT, indicating a breakdown of `sum rules of spectral weight', a signature of a strongly correlated system. Such change in spectral weight is possibly linked to the change in hybridization, lattice volume ({\it i.e.,} effective carrier density), and spin degree of freedom in the system that happens across MIT. We find that MIT in this system is strongly correlation-driven where the electron-electron interactions play a pivotal role. Moreover, our results provide a better insight in understanding the electronic structure of strongly correlated systems and highlight the importance of accounting surface effects during interpretation of the physical property data mainly using surface sensitive probes, such as surface resistivity.",2106.08555v1 2022-03-24,Influence of generated defects by Ar-implantation on the thermoelectric properties of ScN,"Nowadays, making thermoelectric materials more efficient in energy conversion is still a challenge. In this work, to reduce the thermal conductivity and thus improve the overall thermoelectric performances, point and extended defects were generated in epitaxial 111-ScN thin films by implantation using argon ions. The films were investigated by structural, optical, electrical, and thermoelectric characterization methods. The results demonstrated that argon implantation leads to the formation of stable defects (up to 750 K operating temperature) were identified as interstitial type defect clusters and so-called argon-vacancy complexes. The insertion of those specific defects induces acceptor-type deep levels in the bandgap yielding to a reduce of the free carrier mobility. With a reduce electrical conductivity, the irradiated sample exhibited higher Seebeck coefficient maintaining the power factor of the film. The thermal conductivity is strongly reduced from 12 to 3 W.m-1.K-1 at 300 K, showing the effect of defects in increasing phonon scattering. Subsequent high temperature annealing, at 1573 K, leads to the progressive evolution of defects: the initial clusters of interstitial evolved to the benefit of smaller clusters and the formation of bubble. Thus, the number of free carriers, the resistivity and the Seebeck coefficient are almost restored but the mobility of the carriers remains low and a 30% drop in thermal conductivity is still effective (8.5 W.m-1.K-1). This study shows that the control defect engineering with defects introduced by irradiation using noble gases in a thermoelectric coating can be an attractive method to enhance the figure of merit of thermoelectric materials.",2203.13227v4 2022-03-29,Dose rate effects in radiation-induced changes to phenyl-based polymeric scintillators,"Results on the effects of ionizing radiation on the signal produced by plastic scintillating rods manufactured by Eljen Technology company are presented for various matrix materials, dopant concentrations, fluors (EJ-200 and EJ-260), anti-oxidant concentrations, scintillator thickness, doses, and dose rates. The light output before and after irradiation is measured using an alpha source and a photomultiplier tube, and the light transmission by a spectrophotometer. Assuming an exponential decrease in the light output with dose, the change in light output is quantified using the exponential dose constant $D$. The $D$ values are similar for primary and secondary doping concentrations of 1 and 2 times, and for antioxidant concentrations of 0, 1, and 2 times, the default manufacturer's concentration. The $D$ value depends approximately linearly on the logarithm of the dose rate for dose rates between 2.2 Gy/hr and 70 Gy/hr for all materials. For EJ-200 polyvinyltoluene-based (PVT) scintillator, the dose constant is approximately linear in the logarithm of the dose rate up to 3400 Gy/hr, while for polystyrene-based (PS) scintillator or for both materials with EJ-260 fluors, it remains constant or decreases (depending on doping concentration) above about 100 Gy/hr. The results from rods of varying thickness and from the different fluors suggest damage to the initial light output is a larger effect than color center formation for scintillator thickness $\leq1$ cm. For the blue scintillator (EJ-200), the transmission measurements indicate damage to the fluors. We also find that while PVT is more resistant to radiation damage than PS at dose rates higher than about 100 Gy/hr for EJ-200 fluors, they show similar damage at lower dose rates and for EJ-260 fluors.",2203.15923v2 2022-04-11,Thermal insulation and heat guiding using nanopatterned MoS2,"In the modern electronics overheating is one of the major reasons for device failure. Overheating causes irreversible damage to circuit components and can also lead to fire, explosions, and injuries. Accordingly, in the advent of 2D material-based electronics, an understanding of their thermal properties in addition to their electric ones is crucial to enable efficient transfer of excess heat away from the electronic components. In this work we propose structures based on free-standing, few-layer, nanopatterned MoS2 that insulate and guide heat in the in-plane direction. We arrive at these designs via a thorough study of the in-plane thermal conductivity as a function of thickness, porosity, and temperature in both pristine and nanopatterned MoS2 membranes. Two-laser Raman thermometry was employed to measure the thermal conductivities of a set of free-standing MoS2 flakes with diameters greater than 20 um and thicknesses from 5 to 40 nm, resulting in values from 30 to 85 W/mK, respectively. After nanopatterning a square lattice of 100-nm diameter holes with a focused ion beam we have obtained a greater than 10-fold reduction of the thermal conductivities for the period of 500 nm and values below 1 W/mK for the period of 300 nm. The results were supported by equilibrium molecular dynamic simulations for both pristine and nanopatterned MoS2. The selective patterning of certain areas results in extremely large difference in thermal conductivities within the same material. Exploitation of this effect enabled for the first time thermal insulation and heat guiding in the few-layer MoS2. The patterned regions act as high thermal resistors: we obtained a thermal resistance of 4x10-6 m2K/W with only four patterned lattice periods of 300 nm, highlighting the significant potential of MoS2 for thermal management applications.",2204.04999v1 2022-08-04,"Epitaxial growth, magnetoresistance, and electronic band structure of GdSb magnetic semimetal films","Motivated by observations of extreme magnetoresistance (XMR) in bulk crystals of rare-earth monopnictide (RE-V) compounds and emerging applications in novel spintronic and plasmonic devices based on thin-film semimetals, we have investigated the electronic band structure and transport behavior of epitaxial GdSb thin films grown on III-V semiconductor surfaces. The Gd3+ ion in GdSb has a high spin S=7/2 and no orbital angular momentum, serving as a model system for studying the effects of antiferromagnetic order and strong exchange coupling on the resulting Fermi surface and magnetotransport properties of RE-Vs. We present a surface and structural characterization study mapping the optimal synthesis window of thin epitaxial GdSb films grown on III-V lattice-matched buffer layers via molecular beam epitaxy. To determine the factors limiting XMR in RE-V thin films and provide a benchmark for band structure predictions of topological phases of RE-Vs, the electronic band structure of GdSb thin films is studied, comparing carrier densities extracted from magnetotransport, angle-resolved photoemission spectroscopy (ARPES), and density functional theory (DFT) calculations. ARPES shows hole-carrier rich topologically-trivial semi-metallic band structure close to complete electron-hole compensation, with quantum confinement effects in the thin films observed through the presence of quantum well states. DFT predicted Fermi wavevectors are in excellent agreement with values obtained from quantum oscillations observed in magnetic field-dependent resistivity measurements. An electron-rich Hall coefficient is measured despite the higher hole carrier density, attributed to the higher electron Hall mobility. The carrier mobilities are limited by surface and interface scattering, resulting in lower magnetoresistance than that measured for bulk crystals.",2208.02648v2 2023-03-07,"Response to ""On the giant deformation and ferroelectricity of guanidinium nitrate"" by Marek Szafrański and Andrzej Katrusiak","Following a well-established practice of publishing commentaries to articles of other authors who work on materials that were earlier studied by them (n.b. six published comments[1-6]), Marek Szafra\'nski(MS) and Andrzej Katrusiak (AK) have filed on the preprint server arXiv a manuscript entitled ""On the giant deformation and ferroelectricity of guanidinium nitrate""[7] with comments on our article ""Exceptionally high work density of a ferroelectric dynamic organic crystal around room temperature"" published in Nature Communications (2022, 13, 2823).[8] Both in the submitted comment as well as in the required (by the journal) direct communication with us preceding its posting, MS and AK have expressed dissatisfaction with the choice of literature references in our article, for which they felt that their previous work on this material has not been cited to a sufficient extent. In their comment, they summarize their other remarks on our article as ""the structural determinations of GN [guanidinium nitrate] crystals, their phase transitions and associated giant deformation, as well as its detailed structural mechanism, the molecular dynamics and dielectric properties were reported before, while the semiconductivity, ferroelectricity, and fatigue resistance of the GN [guanidinium nitrate] crystals cannot be confirmed.""[7] Apart from the sentiments of MS and AK on our choice of cited literature, we find their comments on the scientific content of our article to be strongly biased towards their own results and unfounded. Below, we provide a detailed response to their comments.",2303.04028v2 2023-05-12,Automated Grain Boundary (GB) Segmentation and Microstructural Analysis in 347H Stainless Steel Using Deep Learning and Multimodal Microscopy,"Austenitic 347H stainless steel offers superior mechanical properties and corrosion resistance required for extreme operating conditions such as high temperature. The change in microstructure due to composition and process variations is expected to impact material properties. Identifying microstructural features such as grain boundaries thus becomes an important task in the process-microstructure-properties loop. Applying convolutional neural network (CNN) based deep-learning models is a powerful technique to detect features from material micrographs in an automated manner. Manual labeling of the images for the segmentation task poses a major bottleneck for generating training data and labels in a reliable and reproducible way within a reasonable timeframe. In this study, we attempt to overcome such limitations by utilizing multi-modal microscopy to generate labels directly instead of manual labeling. We combine scanning electron microscopy (SEM) images of 347H stainless steel as training data and electron backscatter diffraction (EBSD) micrographs as pixel-wise labels for grain boundary detection as a semantic segmentation task. We demonstrate that despite producing instrumentation drift during data collection between two modes of microscopy, this method performs comparably to similar segmentation tasks that used manual labeling. Additionally, we find that na\""ive pixel-wise segmentation results in small gaps and missing boundaries in the predicted grain boundary map. By incorporating topological information during model training, the connectivity of the grain boundary network and segmentation performance is improved. Finally, our approach is validated by accurate computation on downstream tasks of predicting the underlying grain morphology distributions which are the ultimate quantities of interest for microstructural characterization.",2305.07790v1 2011-05-22,Optimal Three-Material Wheel Assemblage of Conducting and Elastic Composites,"We describe a new type of three material microstructures which we call wheel assemblages, that correspond to extremal conductivity and extremal bulk modulus for a composite made of two materials and an ideal material. The exact lower bounds for effective conductivity and matching laminates was found in (Cherkaev, 2009) and for anisotropic composites, in (Cherkaev, Zhang, 2011). Here, we show different optimal structures that generalize the classical Hashin-Shtrikman coated spheres (circles). They consist of circular inclusions which contain a solid central circle (hub) and radial spikes in a surrounding annulus, and (for larger volume fractions of the best material) an annulus filled with it. The same wheel assemblages are optimal for the pair of dual problems of minimal conductivity (resistivity) of a composite made from two materials and an ideal conductor (insulator), in the problem of maximal effective bulk modulus of elastic composites made from two linear elastic material and void, and the dual minimum problem.",1105.4302v1 2015-10-10,Intrusion in heterogeneous materials: Simple global rules from complex micro-mechanics,"The interaction of intruding objects with deformable materials is a common phenomenon, arising in impact and penetration problems, animal and vehicle locomotion, and various geo-space applications. The dynamics of arbitrary intruders can be simplified using Resistive Force Theory (RFT), an empirical framework originally used for fluids but works surprisingly well, better in fact, in granular materials. That such a simple model describes behavior in dry grains, a complex nonlinear material, has invigorated a search to determine the underlying mechanism of RFT. We have discovered that a straightforward friction-based continuum model generates RFT, establishing a link between RFT and local material behavior. Our theory reproduces experimental RFT data without any parameter fitting and generates RFT's key simplifying assumption: a geometry-independent local force formula. Analysis of the system explains why RFT works better in grains than in viscous fluids, and leads to an analytical criterion to predict RFT's in other materials.",1510.02966v1 2017-06-05,Dy$^{3+}$-doped Yttrium Complex Molecular Crystals for Two-color Thermometry in Heterogeneous Materials,"We develop Dy$^{3+}$-doped yttrium complexes for use as two-color thermometry (TCT) phosphor molecular crystals in heterogeneous materials. These complexes include: Dy:Y(acac)$_3$(phen), Dy:Y(hfa)$_3$(DPEPO), Dy:Y(4-BBA)$_3$(TPPO), Dy:Y(acac)$_3$, and Dy:Y(acac)$_3$(DPEPO), where the Dy/Y ratio is 1:9. We characterize the materials' photoluminescence at different temperatures to determine the TCT calibration parameters and the degree to which thermal quenching influences the emission. From this data we observe a link between the excited state lifetime at room temperature and the degree to which the material is susceptible to thermal quenching (i.e. materials having long room temperature lifetimes are more resistant to thermal quenching than materials with short room temperature lifetimes). Of the five complexes tested we find that Dy:Y(acac)$_3$(DPEPO) has the best thermal performance, with the most likely source of improvement being DPEPO's compact rigid structure. This rigidity helps with energy transfer to the Dy$^{3+}$ ion, suppresses non-radiative loss modes, and reduces exciplex formation.",1706.02658v1 1999-12-21,Three-dimensional spontaneous magnetic reconnection in neutral current sheets,"Magnetic reconnection in an antiparallel uniform Harris current sheet equilibrium, which is initially perturbed by a region of enhanced resistivity limited in all three dimensions, is investigated through compressible magnetohydrodynamic simulations. Variable resistivity, coupled to the dynamics of the plasma by an electron-ion drift velocity criterion, is used during the evolution. A phase of magnetic reconnection amplifying with time and leading to eruptive energy release is triggered only if the initial perturbation is strongly elongated in the direction of current flow or if the threshold for the onset of anomalous resistivity is significantly lower than in the corresponding two-dimensional case. A Petschek-like configuration is then built up for \sim 100 Alfven times, but remains localized in the third dimension. Subsequently, a change of topology to an O-line at the center of the system (``secondary tearing'') occurs. This leads to enhanced and time-variable reconnection, to a second pair of outflow jets directed along the O-line, and to expansion of the reconnection process into the third dimension. High parallel current density components are created mainly near the region of enhanced resistivity.",9912443v1 2007-03-05,MHD simulations of jet acceleration from Keplerian accretion disks: the effects of disk resistivity,"Accretion disks and astrophysical jets are used to model many active astrophysical objects, viz., young stars, relativistic stars, and active galactic nuclei. In this paper we present self-consistent time-dependent simulations of supersonic jets launched from magnetized accretion disks, using high resolution numerical techniques. In particular we study the effects of the disk magnetic resistivity, parametrized through an alpha-prescription, in determining the properties of the inflow-outflow system. Moreover we analyze under which conditions steady state solutions of the type proposed in the self similar models of Blandford and Payne can be reached and maintained in a self consistent nonlinear stage. We use the resistive MHD FLASH code with adaptive mesh refinement, allowing us to follow the evolution of the structure for a time scale long enough to reach steady state. A detailed analysis of the initial configuration state is given. We obtain the expected solutions in the axisymmetric (2.5D) limit. Assuming a magnetic field around equipartition with the thermal pressure of the disk, we show how the characteristics of the disk jet system, as the ejection efficiency and the energetics, are affected by the anomalous resistivity acting inside the disk.",0703064v1 1994-09-13,Mesoscopic quantum transport: Resonant tunneling in the presence of strong Coulomb interaction,"Coulomb blockade phenomena and quantum fluctuations are studied in mesoscopic metallic tunnel junctions with high charging energies. If the resistance of the barriers is large compared to the quantum resistance, transport can be described by sequential tunneling. Here we study the influence of quantum fluctuations. They are important when the resistance is small or the temperature very low. A real-time approach is developed which allows the diagrammatic classification of ``inelastic resonant tunneling'' processes where different electrons tunnel coherently back and forth between the leads and the metallic island. With the help of a nonperturbative resummation technique we evaluate the spectral density which describes the charge excitations of the system. From it physical quantities of interest like current and average charge can be deduced. Our main conclusions are: An energy renormalization leads to a logarithmic temperature dependence of the renormalized system parameters. A finite lifetime broadening can change the classical picture drastically. It gives rise to a strong flattening of the Coulomb oscillations for low resistances, but in the Coulomb blockade regime inelastic electron cotunneling persists. The temperature where these effects are important are accessible in experiments.",9409051v1 1994-12-22,"""Scaling of an anomalous metal/insulator transition in a 2D system in silicon at zero magnetic field""","We have studied the temperature dependence of resistivity, $\rho$, for a two-dimensional electron system in silicon at low electron densities, $n_s\sim10^{11}$ cm$^{-2}$, near the metal/insulator transition. The resistivity was empirically found to scale with a single parameter, $T_0$, which approaches zero at some critical electron density, $n_c$, and increases as a power $T_0\propto|n_s-n_c|^\beta$ with $\beta=1.6\pm0.1$ both in metallic ($n_s>n_c$) and insulating ($n_s= 75 T for x = 0.05. This is reminiscent of the composition dependence in high-Tc cuprates and might correlate with opening of a pseudo-gap in the underdoped region. Further, the temperature dependence of Hc2(T) for superconducting samples can be understood in terms of multi-band superconductivity. Rxy data for non-superconducting samples show non-linear field dependence, which is also consistent with a multi-carrier scenario.",0809.1133v3 2008-10-21,Nonlinear resistance of 2D electrons in crossed electric and magnetic fields,"The longitudinal resistivity of two dimensional (2D) electrons placed in strong magnetic field is significantly reduced by applied electric field, an effect which is studied in a broad range of magnetic fields and temperatures in GaAs quantum wells with high electron density. The data are found to be in good agreement with theory, considering the strong nonlinearity of the resistivity as result of non-uniform spectral diffusion of the 2D electrons. Inelastic processes limit the diffusion. Comparison with the theory yields the inelastic scattering time of the two dimensional electrons. In the temperature range T=2-10(K) for overlapping Landau levels, the inelastic scattering rate is found to be proportional to T^2, indicating a dominant contribution of the electron-electron scattering to the inelastic relaxation. In a strong magnetic field, the nonlinear resistivity demonstrates scaling behavior, indicating a specific regime of electron heating of well-separated Landau levels. In this regime the inelastic scattering rate is found to be proportional to T^3, suggesting the electron-phonon scattering as the dominant mechanism of the inelastic relaxation.",0810.3713v2 2008-11-26,Temperature Dependence of Interlayer Magnetoresistance in Anisotropic Layered Metals,"Studies of interlayer transport in layered metals have generally made use of zero temperature conductivity expressions to analyze angle-dependent magnetoresistance oscillations (AMRO). However, recent high temperature AMRO experiments have been performed in a regime where the inclusion of finite temperature effects may be required for a quantitative description of the resistivity. We calculate the interlayer conductivity in a layered metal with anisotropic Fermi surface properties allowing for finite temperature effects. We find that resistance maxima are modified by thermal effects much more strongly than resistance minima. We also use our expressions to calculate the interlayer resistivity appropriate to recent AMRO experiments in an overdoped cuprate which led to the conclusion that there is an anisotropic, linear in temperature contribution to the scattering rate and find that this conclusion is robust.",0811.4442v1 2009-03-04,"Resistivity Anisotropy of $AE$Fe$_2$As$_2$ ($AE$ =Ca, Sr, Ba): direct versus Montgomery technique measurements","The anisotropy of electrical resistivity was measured in parent compounds of the iron-arsenic high temperature superconductors, AEFe2As2 with Alkali Earth elements AE=Ca,Sr, Ba. Measurements were performed using both the Montgomery technique and direct resistivity measurements on samples cut along principal crystallographic directions. The anisotropy ratio \gamma_\rho=\rho_c/\rho_a is well below 10 for all compounds in the whole temperature range studied (4 to 300 K), in notable contrast to previous reports. The anisotropy at room temperature increases from about 2 in Ca, to about 4 in Sr and Ba. In all compounds the resistivity ratio decreases on cooling through the structural/antiferromagnetic transition temperature T_{SM}, with the change mainly coming from stronger variation in \rho_a as compared with \rho_c. This suggests that the transitions stronger affect the two-dimensional parts of the Fermi surface. We compare our experimental observations with band structure calculations, and find similar trend in the evolution of anisotropy with the size of AE ion. Our results show that the electronic structure of the iron pnictides has large contribution from three-dimensional areas of the Fermi surface.",0903.0820v1 2010-04-22,Studies of resistance switching effects in metal/YBa2Cu3O7-x interface junctions,"Current-voltage characteristics of planar junctions formed by an epitaxial c-axis oriented YBa2Cu3O7-x thin film micro-bridge and Ag counter-electrode were measured in the temperature range from 4.2 K to 300 K. A hysteretic behavior related to switching of the junction resistance from a high-resistive to a low-resistive state and vice-versa was observed and analyzed in terms of the maximal current bias and temperature dependence. The same effects were observed on a sub-micrometer scale YBa2Cu3O7-x thin film - PtIr point contact junctions using Scanning Tunneling Microscope. These phenomena are discussed within a diffusion model, describing an oxygen vacancy drift in YBa2Cu3O7-x films in the nano-scale vicinity of the junction interface under applied electrical fields.",1004.3909v1 2010-06-11,Mottness Collapse and T-linear Resistivity in Cuprate Superconductors,"Central to the normal state of cuprate high-temperature superconductors is the collapse of the pseudogap, briefly reviewed here, at a critical point and the subsequent onset of the strange-metal characterized by a resistivity that scales linearly with temperature. A possible clue to the resolution of this problem is the inter-relation between two facts: 1) A robust theory of T-linear resistivity resulting from quantum criticality requires an additional length scale outside the standard 1-parameter scaling scenario and 2) breaking the Landau correspondence between the Fermi gas and an interacting system with short-range repulsions requires non-fermionic degrees. We show that a low-energy theory of the Hubbard model which correctly incorporates dynamical spectral weight transfer has the extra degrees of freedom needed to describe this physics. The degrees of freedom that mix into the lower band as a result of dynamical spectral weight transfer are shown to either decouple beyond a critical doping, thereby signaling Mottness collapse or unbind above a critical temperature yielding strange metal behaviour characterised by $T-$linear resistivity.",1006.2396v1 2011-01-04,The effect of varying Fe-content on transport properties of K intercalated iron selenide KxFe2-ySe2,"We report the successful growth of high-quality single crystals of potassium intercalated iron selenide KxFe2-ySe2 by Bridgeman method. The effect of iron vacancies on transport properties was investigated by electrical resistivity and magnetic susceptibility measurements. With varying iron content, the system passes from semiconducting/insulating to superconducting state. Comparing with superconductivity, the anomalous ""hump"" effect in the normal state resistivity is much more sensitive to the iron deficiency. The electrical resistivity exhibits a perfect metallic behavior (R300K/R35K=42) for the sample with little iron vacancies. Our results suggest that the anomalous ""hump"" effect in the normal state resistivity may be due to the ordering process of the cation vacancies in this non-stoichiometric compound rather than magnetic/structure transition. A trace of superconductivity extending up to near 44 K was also detected in some crystals of KxFe2-ySe2, which has the highest Tc of the reported iron selenides.",1101.0789v1 2011-02-11,Enhancement of edge channel transport by a low frequency irradiation,"The magnetotransport properties of high mobility two dimensional electron gas have recently attracted a significant interest due to the discovery of microwave induced zero resistance states. Here we show experimentally that microwave irradiation with a photon energy much smaller than the spacing between Landau levels can induce a strong decrease in the four terminal resistance. This effect is not predicted by the bulk transport models introduced to explain zero resistance states, but can be naturally explained by an edge transport model. This highlights the importance of edge channels for zero resistance state physics that was proposed recently.",1102.2314v2 2011-05-11,"Systematics of the temperature-dependent inter-plane resistivity in Ba(Fe$_{1-x}$T$_x$)$_2$As$_2$ with T= Rh, Ni, and Pd","Temperature-dependent inter-plane resistivity, $\rho_c(T)$, was measured systematically as a function of transition metal substitution in the iron-arsenide superconductors Ba(Fe$_{1-x}$T$_x$)$_2$As$_2$, $T$= Ni, Pd, Rh. The data are compared with the behavior found in Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$, revealing resistive signatures of pseudogap. In all compounds we find resistivity crossover at a characteristic pseudogap temperature $T^*$ from non-metallic to metallic temperature dependence on cooling. Suppression of $T^*$ proceeds very similar in cases of Ni and Pd doping and much faster than in similar cases of Co and Rh doping. In cases of Co and Rh doping an additional minimum in the temperature-dependent $\rho_c$ emerges for high dopings, when superconductivity is completely suppressed. These features are consistent with the existence of a charge gap covering part of the Fermi surface. The part of the Fermi surface affected by this gap is notably larger for Ni and Pd doped compositions than in Co and Rh doped compounds.",1105.2277v1 2011-09-08,Group velocity and causality in standard relativistic resistive magnetohydrodynamics,"Group velocity of electromagnetic waves in plasmas derived by standard relativistic resistive MHD (resistive RMHD) equations is superluminal. If we assume that the group velocity represents the propagation velocity of a signal, we have to worry about the causality problem. That is, some acausal phenomena may be induced, such that information transportation to the absolute past and spontaneous decrease in the entropy. Here, we tried to find the acausal phenomena using standard resistive RMHD numerical simulations in the suggested situation of the acausal phenomena. The calculation results showed that even in such situations no acausal effect happens. The numerical result with respect to the velocity limit of the information transportation is consistent with a linear theory of wave train propagation. Our results assure that we can use these equations without problems of acausal phenomena.",1109.1856v1 2012-04-03,Resistive and magnetized accretion flows with convection,"We considered the effects of convection on the radiatively inefficient accretion flows (RIAF) in the presence of resistivity and toroidal magnetic field. We discussed the effects of convection on transports of angular momentum and energy. We established two cases for the resistive and magnetized RIAFs with convection: assuming the convection parameter as a free parameter and using mixing-length theory to calculate convection parameter. A self-similar method was used to solve the integrated equations that govern the behavior of the presented model. The solutions showed that the accretion and rotational velocities decrease by adding the convection parameter, while the sound speed increases. Moreover, by using mixing-length theory to calculate convection parameter, we found that the convection can be important in RIAFs with magnetic field and resistivity.",1204.0743v1 2012-08-17,Cooperative dynamics in charge-ordered state of alpha-(BEDT-TTF)2I3,"Electric-field-dependent pulse measurements are reported in the charge-ordered state of alpha-(BEDT-TTF)2I3. At low electric fields up to about 50 V/cm only negligible deviations from Ohmic behavior can be identified with no threshold field. At larger electric fields and up to about 100 V/cm a reproducible negative differential resistance is observed with a significant change in shape of the measured resistivity in time. These changes critically depend whether constant voltage or constant current is applied to the single crystal. At high enough electric fields the resistance displays a dramatic drop down to metallic values and relaxes subsequently in a single-exponential manner to its low-field steady-state value. We argue that such an electric-field induced negative differential resistance and switching to transient states are fingerprints of cooperative domain-wall dynamics inherent to two-dimensional bond-charge density wave with ferroelectric-like nature.",1208.3609v2 2012-11-05,Metastable Resistivity States and Conductivity Fluctuations in Low-doped La$_{1-x}$Ca$_{x}$MnO$_3$ Manganite Single Crystals,"Conductivity noise in dc current biased La_{0.82}Ca_{0.18}MnO_{3} single crystals has been investigated in different metastable resistivity states enforced by applying voltage pulses to the sample at low temperatures. Noise measured in all investigated resistivity states is of 1/f-type and its intensity at high temperatures and low dc bias scales as a square of the bias. At liquid nitrogen temperatures for under bias exceeding a threshold value, the behavior of the noise deviates from above quasi- equilibrium modulation noise and depends in a non monotonic way on applied bias. The bias range of nonequilibrium 1/f noise coincides with the range at which the conductance increases linearly with bias voltage. This feature is attributed to a broad continuity of states enabling indirect inelastic tunneling across intrinsic tunnel junctions. The nonequilibrium noise has been ascribed to indirect intrinsic tunneling mechanism while resistivity changes in metastable states to variations in the energy landscape for charge carriers introduced by microcracks created by the pulse procedures employed",1211.0838v1 2012-11-07,Exchange Field-Mediated Magnetoresistance in the Correlated Insulator Phase of Be Films,"We present a study of the proximity effect between a ferromagnet and a paramagnetic metal of varying disorder. Thin beryllium films are deposited onto a 5 nm-thick layer of the ferromagnetic insulator EuS. This bilayer arrangement induces an exchange field, $H_{ex}$, of a few tesla in low resistance Be films with sheet resistance $R\ll R_Q$, where $R_Q=h/e^2$ is the quantum resistance. We show that $H_{ex}$ survives in very high resistance films and, in fact, appears to be relatively insensitive to the Be disorder. We exploit this fact to produce a giant low-field magnetoresistance in the correlated insulator phase of Be films with $R\gg R_Q$.",1211.1663v1 2013-04-30,Mechanical resistance in unstructured proteins,"Single-molecule pulling experiments on unstructured proteins linked to neurodegenerative diseases have measured rupture forces comparable to those for stable folded proteins. To investigate the structural mechanisms of this unexpected force resistance, we perform pulling simulations of the amyloid {\beta}-peptide (A{\beta}) and {\alpha}-synuclein ({\alpha}S), starting from simulated conformational ensembles for the free monomers. For both proteins, the simulations yield a set of rupture events that agree well with the experimental data. By analyzing the conformations right before rupture in each event, we find that the mechanically resistant structures share a common architecture, with similarities to the folds adopted by A{\beta} and {\alpha}S in amyloid fibrils. The disease-linked Arctic mutation of A{\beta} is found to increase the occurrence of highly force-resistant structures. Our study suggests that the high rupture forces observed in A{\beta} and {\alpha}S pulling experiments are caused by structures that might have a key role in amyloid formation.",1304.7991v3 2013-06-11,Effect of pressure cycling on Iron: Signatures of an electronic instability and unconventional superconductivity,"High pressure electrical resistivity and x-ray diffraction experiments have been performed on Fe single crystals. The crystallographic investigation provides direct evidence that in the martensitic $bcc \rightarrow hcp$ transition at 14 GPa the $\lbrace 110\rbrace_{bcc}$ become the $\lbrace 002\rbrace_{hcp}$ directions. During a pressure cycle, resistivity shows a broad hysteresis of 6.5 GPa, whereas superconductivity, observed between 13 and 31 GPa, remains unaffected. Upon increasing pressure an electronic instability, probably a quantum critical point, is observed at around 19 GPa and, close to this pressure, the superconducting $T_{c}$ and the isothermal resistivity ($0B_{th}$), the symmetry is spontaneously broken. At sufficiently high magnetic field and low temperature the model predicts a phase with a non-vanishing permanent current; this is a novel phase that has not been observed so far.",1104.4476v1 2012-03-08,Precision quantization of Hall resistance in transferred graphene,"We show that quantum resistance standards made of transferred graphene reach the uncertainty of semiconductor devices, the current reference system in metrology. A large graphene device (150 \times 30 \mum2), exfoliated and transferred onto GaAs, revealed a quantization with a precision of (-5.1 \pm 6.3) \times 10-9 accompanied by a vanishing longitudinal resistance at current levels exceeding 10 \muA. While such performance had previously only been achieved with epitaxially grown graphene, our experiments demonstrate that transfer steps, inevitable for exfoliated graphene or graphene grown by chemical vapor deposition (CVD), are compatible with the requirements of high quality quantum resistance standards.",1203.1798v2 2012-03-23,Pressure effects on the heavy-fermion antiferromagnet CeAuSb2,"The f-electron compound CeAuSb2, which crystallizes in the ZrCuSi2-type tetragonal structure, orders antiferromagnetically between 5 and 6.8 K, where the antiferromagnetic transition temperature T_N depends on the occupancy of the Au site. Here we report the electrical resistivity and heat capacity of a high-quality crystal CeAuSb2 with T_N of 6.8 K, the highest for this compound. The magnetic transition temperature is initially suppressed with pressure, but is intercepted by a new magnetic state above 2.1 GPa. The new phase shows a dome shape with pressure and coexists with another phase at pressures higher than 4.7 GPa. The electrical resistivity shows a T^2 Fermi liquids behavior in the complex magnetic state, and the residual resistivity and the T^2 resistivity coefficient increases with pressure, suggesting the possibility of a magnetic quantum critical point at a higher pressure.",1203.5164v1 2015-06-03,Electronic resistances of multilayered two-dimensional crystal junctions,"We carry out a layer-by-layer investigation to understand electron transport across metal-insulator-metal junctions. Interfacial structures of junctions were studied and characterized using first-principles density functional theory within the generalized gradient approximation. We found that as a function of the number of crystal layers the calculated transmission coefficients of multilayer silicene junctions decay much slower than for BN-based junctions We revisited the semiclassical Boltzmann theory of electronic transport and applied to multilayer silicene and BN-based junctions. The calculated resistance in the high-transmission regime is smaller than that provided by the Landauer formula. As the thickness of the barrier increases, results from the Boltzmann and the Landauer formulae converge. We provide a upper limit in the transmission coefficient below which, the Landauer method becomes valid. Quantitatively, when the transmission coefficient is lower than $ \sim 0.05 $ per channel, the error introduced by the Landauer formula for calculating the resistance is negligible. In addition, we found that the resistance of a junction is not entirely determined by the averaged transmission, but also by the distribution of the transmission over the first Brillouin zone.",1506.01397v1 2019-01-28,Quantifying Temperature-dependent Substrate Loss in GaN-on-Si RF Technology,"Intrinsic limits to temperature-dependent substrate loss for GaN-on-Si technology, due to the change in resistivity of the substrate with temperature, are evaluated using an experimentally validated device simulation framework. Effect of room temperature substrate resistivity on temperature-dependent CPW line loss at various operating frequency bands are then presented. CPW lines for GaN-on-high resistivity Si are shown to have a pronounced temperature-dependence for temperatures above 150{\deg}C and have lower substrate losses for frequencies above the X-band. On the other hand, GaN-on-low resistivity Si is shown to be more temperature-insensitive and have lower substrate losses than even HR-Si for lower operating frequencies. The effect of various CPW geometries on substrate loss is also presented to generalize the discussion. These results are expected to act as a benchmark for temperature dependent substrate loss in GaN-on-Si RF technology.",1901.09521v1 2019-01-29,Simultaneous prediction of multiple outcomes using revised stacking algorithms,"Motivation: HIV is difficult to treat because its virus mutates at a high rate and mutated viruses easily develop resistance to existing drugs. If the relationships between mutations and drug resistances can be determined from historical data, patients can be provided personalized treatment according to their own mutation information. The HIV Drug Resistance Database was built to investigate the relationships. Our goal is to build a model using data in this database, which simultaneously predicts the resistance of multiple drugs using mutation information from sequences of viruses for any new patient. Results: We propose two variations of a stacking algorithm which borrow information among multiple prediction tasks to improve multivariate prediction performance. The most attractive feature of our proposed methods is the flexibility with which complex multivariate prediction models can be constructed using any univariate prediction models. Using cross-validation studies, we show that our proposed methods outperform other popular multivariate prediction methods. Availability: An R package will be made available.",1901.10153v1 2019-06-07,A resistive extension for ideal MHD,"We present an extension to the special relativistic, ideal magnetohydrodynamics (MHD) equations, designed to capture effects due to resistivity. The extension takes the simple form of an additional source term which, when implemented numerically, is shown to emulate the behaviour produced by a fully resistive MHD description for a range of initial data. The extension is developed from first principle arguments, and thus requires no fine tuning of parameters, meaning it can be applied to a wide range of dynamical systems. Furthermore, our extension does not suffer from the same stiffness issues arising in resistive MHD, and thus can be evolved quickly using explicit methods, with performance benefits of roughly an order of magnitude compared to current methods.",1906.03150v2 2019-06-19,Phonon scattering induced carrier resistivity in twisted double bilayer graphene,"In this work we carry out a theoretical study of the phonon-induced resistivity in twisted double bilayer graphene (TDBG), in which two Bernal-stacked bilayer graphene devices are rotated relative to each other by a small angle $\theta$. We show that at small twist angles ($\theta\sim 1^\circ$) the effective mass of the TDBG system is greatly enhanced, leading to a drastically increased phonon-induced resistivity in the high-temperature limit where phonon scattering leads to a linearly increasing resistivity with increasing temperature. We also discuss possible implications of our theory on superconductivity in such a system, and provide an order of magnitude estimation of the superconducting transition temperature.",1906.08224v2 2021-02-16,Fast hierarchical inversion for borehole resistivity measurements in high-angle and horizontal wells using ADNN-AMLM,"With the rapid development of deep learning, intelligent scheme is gradually introduced to solve various nolinear inverse problems. In this paper, we combine an efficient adaptive deep neural network (ADNN) framework with adaptive modified Levenberg-Marquardt (AMLM) algorithm based on three-layer inversion model to exact formation resistivity and invasion depth from array laterolog resistivity measurements. ADNN presented in this paper can realize the 2D/3D fast forward modeling of array laterolog. AMLM algorithm and hierarchical inversion scheme are adopted to improve the anti-noise ability and convergence in complex logging environments, which realizing the fast and accurate reconstruction of longitudinal resistivity profile in HA/HZ wells. The numerical simulation shows that the ADNN forward modeling only takes 0.021s for each logging point, and the maximum relative error is less than 2%. Three-layer inversion model can eliminate the effect of surrounding bed and improve the inversion accuracy in thinly layered formation. The error between inverted results and truth model is less than 3%. The AMLM inversion algorithm can effectively suppress the influence of noise, and takes only 10 steps to achieve convergence.",2102.08038v1 2021-04-01,Towards high-rate RPC-based thermal neutron detectors using low-resistivity electrodes,"We present experimental results on the counting rate measurements for several single-gap $^{10}$B lined resistive plate chambers ($^{10}$B-RPCs) with anodes made from standard float glass, low resistivity glass and ceramic. The measurements were performed at the V17 monochromatic neutron beamline (3.35 \.A) at the Helmholtz-Zentrum Berlin. For the $^{10}$B-RPCs with 0.28 mm thick float glass a maximum counting rate density of about $8\times 10^{3}$ $Hz/cm^{2}$ was obtained. In the case of low resistivity glass and ceramic, the counting rate density did not deviate from linear dependence on the neutron flux up to the maximum flux available at this beamline and exceeded a value of $3\times 10^{4}$ $Hz/cm^{2}$.",2104.00695v1 2021-09-14,Contactless Series Resistance Imaging of Perovskite Solar Cells via Inhomogeneous Illumination,"A contactless effective series resistance imaging method for large area perovskite solar cells that is based on photoluminescence imaging with non-uniform illumination is introduced and demonstrated experimentally. The proposed technique is applicable to partially and fully processed perovskite solar cells if laterally conductive layers are present. The capability of the proposed contactless method to detect features with high effective series resistance is validated by comparison with various contacted mode luminescence imaging techniques. The method can reliably provide information regarding the severeness of the detected series resistance through photo-excitation pattern manipulation. Application of the method to sub-cells in monolithic tandem devices, without the need for electrical contacting the terminals, appears feasible.",2109.06971v1 2021-12-29,Wide-range $T^2$ resistivity and umklapp scattering in moiré graphene,"We argue that the unusually strong electron-electron interactions in the narrow bands in moir\'e superlattices originate from compact Wannier orbitals. Enhanced overlaps of electronic wavefunctions, enabled by such orbitals, result in a strong el-el superlattice umklapp scattering. We identify the umklapp scattering processes as a source of the strong temperature-dependent resistivity observed in these systems. In a simple model, the umklapp scattering predicts a $T$-dependent resistivity that grows as $T^2$ and is getting bigger as the Wannier orbital radius decreases. We quantify the enhancement in el-el scattering by the Kadowaki-Woods (KW) ratio, a quantity that is sensitive to umklapp scattering but, helpfully, insensitive to the effects due to the high density of electronic states. Our analysis predicts anomalously large KW ratio values that clearly indicate the importance of the umklapp el-el processes and their impact on the $T$-dependent resistivity.",2112.14745v2 2022-06-05,Simplicial effective resistance and enumeration of spanning trees,"A graph can be regarded as an electrical network in which each edge is a resistor. This point of view relates combinatorial quantities, such as the number of spanning trees, to electrical ones such as effective resistance. The second and third authors have extended the combinatorics/electricity analogy to higher dimension and expressed the simplicial analogue of effective resistance as a ratio of weighted tree enumerators. In this paper, we first use that ratio to prove a new enumeration formula for color-shifted complexes, confirming a conjecture by Aalipour and the first author, and generalizing a result of Ehrenborg and van Willigenburg on Ferrers graphs. We then use the same technique to recover an enumeration formula for shifted complexes, first proved by Klivans and the first and fourth authors. In each case, we add facets one at a time, and give explicit expressions for simplicial effective resistances of added facets by constructing high-dimensional analogues of currents and voltages (respectively homological cycles and cohomological cocycles).",2206.02182v2 2022-11-25,Numerical study of SQUID array responses due to asymmetric junction parameters,"Superconducting quantum interference device arrays have been extensively studied for their high magnetic field sensitivity. The performance of these devices strongly depends on the characteristic parameters of their Josephson junctions, i.e. their critical currents and shunt resistances. Using a resistively shunted junction model and including thermal noise, we perform a numerical investigation of the effects of asymmetric Josephson junctions by independently studying variations in the critical currents and junction resistances. We compare the voltage response of a dc-SQUID with a 1D parallel SQUID array and study the maximum transfer function dependence on the number of junctions in parallel, the screening parameter and thermal noise strength. Our results show that the maximum transfer function and linearity increase with the number of junctions in parallel for arrays with different junction resistances, in contrast to SQUID arrays with identical junctions or with spreads in the critical currents.",2211.13833v1 2023-01-08,Resistive Read-out in Thin Silicon Sensors with Internal Gain,"Two design innovations, low-gain avalanche (Low-Gain Avalance Diode, LGAD) and resistive read-out (Resistive Silicon Detector, RSD), have brought strong performance improvements to silicon sensors. Large signals, due to the added gain mechanism, lead to improved temporal precision, while charge sharing, introduced by resistive read-out, allows for achieving excellent spatial resolution even with large pixels. LGAD- and RSD- based silicon sensors are now adopted, or considered, in several future experiments and are the basis for almost every next 4D-trackers. New results obtained with sensors belonging to the second FBK production of RSD (RSD2) demonstrate how a combined resolution of 30 ps and 30 \microns can be obtained with pixels as large as $1 \times 1 $ mm$^2$.",2301.02968v1 2023-06-09,Voltage-time dilemma and stochastic threshold voltage variation in pure silver atomic switches,"The formation and dissolution of silver nanowires plays a fundamental role in a broad range of resistive switching devices, fundamentally relying on the electrochemical metallization phenomenon. It was shown, however, that resistive switching may also appear in pure metallic nanowires lacking any silver-ion-hosting embedding environment, but this pure atomic switching mechanism fundamentally differs from the conventional electrochemical-metallization-based resistive switching. To facilitate the quantitative description of the former phenomenon, we investigate broad range of Ag atomic junctions with a special focus on the frequency-dependence and the fundamentally stochastic cycle-to-cycle variation of the switching threshold voltage. These devices are established in an ultra-high purity environment where electrochemical metallization can be excluded. The measured characteristics are successfully described by a vibrational pumping model, yielding consistent predictions for the weak frequency dependence and the large variance of the switching threshold voltage. We also demonstrate that electrochemical-metallization-based resistive switching and pure atomic switching may appear in the same device structure, and therefore the proper understanding of the pure atomic switching mechanism has a distinguished importance in silver-based electrochemical metallization cells.",2306.05736v1 2023-08-19,"Temperature, RF Field, and Frequency Dependence Performance Evaluation of Superconducting Niobium Half-Wave Cavity","Recent advancement in superconducting radio frequency cavity processing techniques, with diffusion of impurities within the RF penetration depth, resulted in high quality factor with increase in quality factor with increasing accelerating gradient. The increase in quality factor is the result of a decrease in the surface resistance as a result of nonmagnetic impurities doping and change in electronic density of states. The fundamental understanding of the dependence of surface resistance on frequency and surface preparation is still an active area of research. Here, we present the result of RF measurements of the TEM modes in a coaxial half wave niobium cavity resonating at frequencies between 0.3-1.3 GHz. The temperature dependence of the surface resistance was measured between 4.2 K and 1.6 K. The field dependence of the surface resistance was measured at 2.0 K. The baseline measurements were made after standard surface preparation by buffered chemical polishing.",2308.09859v1 2023-12-16,Negative differential resistance in Josephson junctions coupled to a cavity,"Regions with negative differential resistance can arise in the IV curve of Josephson junctions and this phenomenon plays an essential role for applications, in particular for THz radiation emission. For the measurement of high frequency radiation from Josephson junctions, a cavity - either internal or external - is often used. A cavity may also induce a negative differential resistance region at the lower side of the resonance frequency. We investigate the dynamics of Josephson junctions with a negative differential resistance in the quasi particle tunnel current, i.e. in the McCumber curve. We find that very complicated and unexpected interactions take place. This may be useful for the interpretation of experimental measurements of THz radiation from intrinsic Josephson junctions.",2312.14174v1 1995-01-26,Superconductivity and Stoichiometry in the BSCCO-family Materials,"We report on magnetization, c-axis and ab-plane resistivity, critical current, electronic band structure and superconducting gap properties. Bulk measurements and photoemission data were taken on similar samples.",9501124v1 2002-06-14,Electron scattering in multi-wall carbon-nanotubes,"We analyze two scattering mechanisms that might cause intrinsic electronic resistivity in multi-wall carbon nanotubes: scattering by dopant impurities, and scattering by inter-tube electron-electron interaction. We find that for typically doped multi-wall tubes backward scattering at dopants is by far the dominating effect.",0206264v1 2003-07-11,Magnetic and transport percolation in diluted magnetic semiconductors,"The ferromagnetic transition in a diluted magnetic semiconductor with localized charge carriers is inevitably a percolation transition. In this work we theoretically study the correlation between this magnetic percolation and transport properties of the sample, including the possibility of a simultaneous transport percolation. We find nontrivial signatures of the percolating magnetic clusters in the transport properties of the system, including interesting non-monotonic temperature dependence of the system resistivity.",0307294v1 2003-09-26,Vortex dynamics in dilute two dimensional Josephson junction arrays,"We have investigated the dynamics of vortices in a dilute two dimensional Josephson junction array where a fraction of the superconducting islands is missing. We have used the multiple trapping model to calculate the mobility of vortices and the frequency dependence of the resistance and inductance of the array.",0309620v1 2004-04-01,Hall anomaly in mixed state of superconductors and vortex dynamics,"The present author has long argued, with concrete predictions, that both longitudinal and transverse (Hall) resistivities in the mixed state of superconductors are dominated by vortex many-body effect. Hence there is no need to introduce various ad hoc vortex dynamics theories. It is interesting to note this point of view is now slowly creeping into the work of his most fierce opponents.",0404009v1 2010-01-29,Cooper pairs under the action of disorder and strong magnetic field,"The zero temperature phase diagram of Cooper pairs exposed to disorder and magnetic field is found to exhibit four distinct phases: a Bose and a Fermi insulating, a metallic and a superconducting phase, respectively. The results explain the giant negative magneto-resistance found experimentally in In-O, TiN, Bi and high-$T_c$ materials.",1001.5431v2 2011-01-17,Localized superconductive pairs,"Different physical phenomena are discussed which should help to comprehend and interpret the concept of localized superconductive pairs; these include behavior of highly resistive granular materials with superconducting grains, parity effect and the Berezinskii--Kosterlitz--Thouless transition. Experimental arguments in support of localized pairs existence are presented and conditions which promote their appearance are analyzed.",1101.3203v2 2016-07-06,Multilayer coating for higher accelerating fields in superconducting radio-frequency cavities: a review of theoretical aspects,"Theory of the superconductor-insulator-superconductor (S-I-S) multilayer structure in superconducting accelerating cavity application is reviewed. The theoretical field limit, optimum layer thicknesses and material combination, and surface resistance are discussed. Those for the S-S bilayer structure are also reviewed.",1607.01495v3 2023-05-25,Structure and properties of the films based on ternary transition metal borides: theory and experiment,"The review presents the results of theoretical and experimental studies of the structure, bonding between atoms, mechanical properties, thermal stability, and oxidation and corrosion resistance of films based on ternary transition metal borides.",2305.15854v1 2005-12-19,Insulating transition in the flux-flow resistivity of a high temperature superconductor,"Measurements of the DC resistivity of under-doped cuprate superconductors have revealed a metal--insulator transition at low temperatures when superconductivity is suppressed by a very large magnetic field, with the resistivity growing logarithmically in the low temperature limit. This insulating behaviour has been associated not only with the large magnetic fields, but also with the under-doped composition and intrinsic sample inhomogeneity, and it is important to establish whether these factors are essential to it. Here we report high resolution microwave measurements of the flux-flow resistivity of optimally doped YBa_(2)Cu_(3)O_(6+x) in the mixed state at temperatures down to 1.2 K. We find that the effective resistivity of the vortex cores exhibits a metal-insulator transition, with a minimum at 13 K and a logarithmically growing form below 5 K. The transition is seen in samples of the highest quality and in magnetic fields as low as 1 T. Our work is the first report of a metal-insulator transition in optimally doped YBa_(2)Cu_(3)O_(6+x), and the first such transition to be seen in a system in which superconductivity has not been globally suppressed.",0512459v1 2010-09-30,Resistivity-driven State Changes in Vertically Stratified Accretion Disks,"We investigate the effect of shear viscosity and Ohmic resistivity on the magnetorotational instability (MRI) in vertically stratified accretion disks through a series of local simulations with the Athena code. First, we use a series of unstratified simulations to calibrate physical dissipation as a function of resolution and background field strength; the effect of the magnetic Prandtl number, Pm = viscosity/resistivity, on the turbulence is captured by ~32 grid zones per disk scale height, H. In agreement with previous results, our stratified disk calculations are characterized by a subthermal, predominately toroidal magnetic field that produces MRI-driven turbulence for |z| < 2 H. Above |z| = 2 H, magnetic pressure dominates and the field is buoyantly unstable. Large scale radial and toroidal fields are also generated near the mid-plane and subsequently rise through the disk. The polarity of this mean field switches on a roughly 10 orbit period in a process that is well-modeled by an alpha-omega dynamo. Turbulent stress increases with Pm but with a shallower dependence compared to unstratified simulations. For sufficiently large resistivity, on the order of cs H/1000, where cs is the sound speed, MRI turbulence within 2 H of the mid-plane undergoes periods of resistive decay followed by regrowth. This regrowth is caused by amplification of toroidal field via the dynamo. This process results in large amplitude variability in the stress on 10 to 100 orbital timescales, which may have relevance for partially ionized disks that are observed to have high and low accretion states.",1010.0005v2 2011-11-30,Self-Similar Solutions for Viscous and Resistive ADAF,"In this paper, the self-similar solution of resistive advection dominated accretion flows (ADAF) in the presence of a pure azimuthal magnetic field is investigated. The mechanism of energy dissipation is assumed to be the viscosity and the magnetic diffusivity due to turbulence in the accretion flow. It is assumed that the magnetic diffusivity and the kinematic viscosity are not constant and vary by position and $\alpha$-prescription is used for them. In order to solve the integrated equations that govern the behavior of the accretion flow, a self-similar method is used. The solutions show that the structure of accretion flow depends on the magnetic field and the magnetic diffusivity. As, the radial infall velocity and the temperature of the flow increase, and the rotational velocity decreases. Also, the rotational velocity for all selected values of magnetic diffusivity and magnetic field is sub-Keplerian. The solutions show that there is a certain amount of magnetic field that the rotational velocity of the flow becomes zero. This amount of the magnetic field depends on the gas properties of the disc, such as adiabatic index and viscosity, magnetic diffusivity, and advection parameters. The solutions show the mass accretion rate increases by adding the magnetic diffusivity and in high magnetic pressure case, the ratio of the mass accretion rate to the Bondi accretion rate decreases as magnetic field increases. Also, the study of Lundquist and magnetic Reynolds numbers based on resistivity indicates that the linear growth of magnetorotational instability (MRI) of the flow decreases by resistivity. This property is qualitatively consistent with resistive magnetohydrodynamics (MHD) simulations.",1111.7302v1 2016-11-09,Numerical integral of resistance coefficients in diffusion,"The resistance coefficients in screen Coulomb potential of stellar plasma are evaluated in high accuracy. I have analyzed the possible singularities in the integral of scattering angle. There are possible singularities in the case of attractive potential. This may result in problem for numerical integral. In order to avoid the problem, I have used a proper scheme, e.g., splitting into many subintervals and the width of each subinterval is determined by the variation of the integrand, to calculate the scattering angle. The collision integrals are calculated by using Romberg's method therefore the accuracy is high (i.e., $ \sim 10^{-12}$). The results of collision integrals and their derivatives in $-12 \leq \psi \leq 5$ are listed. By using Hermite polynomial interpolation from those data, the collision integrals can be obtained with an accuracy of $10^{-10}$. For very weak coupled plasma ($\psi \geq 4.5$), analytical fittings for collision integrals are available with an accuracy of $10^{-11}$. I have compared the final results of resistance coefficients with other works and found that, for repulsive potential, the results are basically same to others, for attractive potential, the results in intermediate and strong coupled case show significant differences. The resulting resistance coefficients are tested in the solar model. Comparing with the widely used Cox et al.(1989) and Thoul et al. (1994) models, the resistance coefficients in screen Coulomb potential leads to a little weaker effect in solar model, which is contrary to the expectation of attempts to solve the solar abundance problem.",1611.03115v1 2019-03-28,Dynamic Streaming Spectral Sparsification in Nearly Linear Time and Space,"In this paper we consider the problem of computing spectral approximations to graphs in the single pass dynamic streaming model. We provide a linear sketching based solution that given a stream of edge insertions and deletions to a $n$-node undirected graph, uses $\tilde O(n)$ space, processes each update in $\tilde O(1)$ time, and with high probability recovers a spectral sparsifier in $\tilde O(n)$ time. Prior to our work, state of the art results either used near optimal $\tilde O(n)$ space complexity, but brute-force $\Omega(n^2)$ recovery time [Kapralov et al.'14], or with subquadratic runtime, but polynomially suboptimal space complexity [Ahn et al.'14, Kapralov et al.'19]. Our main technical contribution is a novel method for `bucketing' vertices of the input graph into clusters that allows fast recovery of edges of sufficiently large effective resistance. Our algorithm first buckets vertices of the graph by performing ball-carving using (an approximation to) its effective resistance metric, and then recovers the high effective resistance edges from a sketched version of an electrical flow between vertices in a bucket, taking nearly linear time in the number of vertices overall. This process is performed at different geometric scales to recover a sample of edges with probabilities proportional to effective resistances and obtain an actual sparsifier of the input graph. This work provides both the first efficient $\ell_2$-sparse recovery algorithm for graphs and new primitives for manipulating the effective resistance embedding of a graph, both of which we hope have further applications.",1903.12150v1 2019-06-20,Substrate mediated nitridation of niobium into superconducting Nb2N thin films for phase slip study,"Here we report a novel nitridation technique for transforming niobium into hexagonal Nb2N which appears to be superconducting below 1K. The nitridation is achieved by high temperature annealing of Nb films grown on Si3N4/Si (100) substrate under high vacuum. The structural characterization directs the formation of a majority Nb2N phase while the morphology shows granular nature of the films. The temperature dependent resistance measurements reveal a wide metal-to-superconductor transition featuring two distinct transition regions. The region close to the normal state varies strongly with the film thickness, whereas, the second region in the vicinity of the superconducting state remains almost unaltered but exhibiting resistive tailing. The current-voltage characteristics also display wide transition embedded with intermediate resistive states originated by phase slip lines. The transition width in current and the number of resistive steps depend on film thickness and they both increase with decrease in thickness. The broadening in transition width is explained by progressive establishment of superconductivity through proximity coupled superconducting nano-grains while finite size effects and quantum fluctuation may lead to the resistive tailing. Finally, by comparing with Nb control samples, we emphasize that Nb2N offers unconventional superconductivity with promises in the field of phase slip based device applications.",1906.08692v1 2021-04-28,Channel Models and Coding Solutions for 1S1R Crossbar Resistive Memory with High Line Resistance,"Crossbar resistive memory with the 1 Selector 1 Resistor (1S1R) structure is attractive for nonvolatile, high-density, and low-latency storage-class memory applications. As technology scales down to the single-nm regime, the increasing resistivity of wordline/bitline becomes a limiting factor to device reliability. This paper presents write/read communication channels while considering the line resistance and device variabilities by statistically relating the degraded write/read margins and the channel parameters. Binary asymmetric channel (BAC) models are proposed for the write/read operations. Simulations based on these models suggest that the bit-error rate of devices are highly non-uniform across the memory array. These models provide quantitative tools for evaluating the trade-offs between memory reliability and design parameters, such as array size, technology nodes, and aspect ratio, and also for designing coding-theoretic solutions that would be most effective for crossbar memory. Method for optimizing the read threshold is proposed to reduce the raw bit-error rate (RBER). We propose two schemes for efficient channel coding based on Bose-Chaudhuri-Hocquenghem (BCH) codes. An interleaved coding scheme is proposed to mitigate the non-uniformity of reliability and a location dependent coding framework is proposed to leverage this non-uniformity. Both of our proposed coding schemes effectively reduce the undetected bit-error rate (UBER).",2104.14011v1 2022-05-13,The Relationship Between Insulin Resistance Neutrophil to Lymphocyte Ratio,"Aim: There is increasing interest in the role of chronic inflammation on pathogenesis of various disease, and one of its markers, high NLR is associated with various mortality and morbidity risk. Insulin resistance (IR) might be one potential associate factors, as suggested in preclinical studies. However, epidemiological studies are scarce which investigated the association between NLR, and insulin resistance (IR) and they included only diabetes mellitus patients, not the general population. This study aims to determine if there is a direct correlation between NLR and IR in the US general population. Methods: The sample consists of 3,307 from general population, provided by National Health and Nutrition Examination Survey (NHANES). Homeostasis Model Assessment of Insulin Resistance (HOMA-IR) value was calculated to evaluate insulin resistance. We investigated the relationship between their NLR and HOMA-IR values by bivariate and multivariate linear regression analyses. As insulin use could results in inaccurate HOMA-IR estimation, we excluded them and ran the analyses in subgroup analyses. Results: There was a relationship shown when insulin users were included, having a beta coefficient value of 0.010 (95% confidence interval [CI] of 0.003-0.017). However, when insulin users were excluded, the beta value decreased to 0.004 (95% CI of -0.006-0.015). The statistical significance was not reached when age, sex, and body mass index were adjusted for in the multivariate analyses. Conclusion: There is no visible relationship between IR and NLR in the general population. IR might not explain the variation of NLR value in healthy people, and further studies are needed to reveal the associated factor of high NLR.",2205.08308v2 2019-12-08,Multifilamentary character of anticorrelated capacitive and resistive switching in memristive structures based on (CoFeB)x(LiNbO3)100-x nanocomposite,"Resistive and capacitive switching in capacitor metal/nanocomposite/metal (M/NC/M) structures based on (CoFeB)x(LiNbO3)100-x NC fabricated by ion-beam sputtering with metal content x $\approx$ 8-20 at. % is studied. The peculiarity of the structure synthesis was the use of increased oxygen content ($\approx$ 2*10^-5 Torr) at the initial stage of the NC growth. The NC films, along with metal nanogranules of 3-6 nm in size, contained a large number of dispersed Co (Fe) atoms (up to ~10^22 cm^-3). Measurements were performed both in DC and AC (frequency range 5-13 MHz) regimes. When switching structures from high-resistance (Roff) to low-resistance (Ron) state, the effect of a strong increase in their capacity was found, which reaches 8 times at x $\approx$ 15 at. % and the resistance ratio Roff/Ron $\approx$ 40. The effect is explained by the synergetic combination of the multifilamentary character of resistive switching (RS) and structural features of the samples associated, in particular, with the formation of high-resistance and strongly polarizable LiNbO3 layer near the bottom electrode of the structures. The proposed model is confirmed by investigations of RS of two-layer nanoscale M/NC/LiNbO3/M structures as well as by studies of the magnetization of M/NC/M structures in the pristine state and after RS.",1912.03726v3 2024-04-17,Stress analysis of functionally graded hyperelastic variable thickness rotating annular thin disk: A semi-analytic approach,"Functionally graded materials (FGMs) represent a promising class of advanced materials designed with tailored microstructures to achieve optimized mechanical, thermal, and functional properties across varying gradients. The strategic integration of distinct materials within functionally graded materials offers engineers unprecedented control over properties such as strength, thermal conductivity, and corrosion resistance, enabling innovative solutions for demanding applications in aerospace, automotive, and biomedical industries. This study investigates a rotating annular thin disk with variable thickness composed of incompressible hyperelastic material, made up of functionally graded properties under large deformations. To elucidate these phenomena, a power relation is employed to delineate the changes in cross-sectional geometry m, the material property n, and the angular velocity w of hyperelastic material. Constants used for hyperelastic material are obtained from the experimental data. Equations are solved semi-analytically for different values of m, n, and w, and the values of radial stresses, tangential stresses, and elongation are calculated and compared for different conditions. Results show that thickness and FG properties have a significant impact on the behavior of disk, so that the expected behavior of the disk can be obtained by an optimal selection of the disks geometry and material properties. By selecting the optimum values for these variables, the location of maximum stress can be controlled in large deformations, thereby furnishing significance advantages in structural design and material selection.",2404.11365v1 2023-05-03,Universal sublinear resistivity in vanadium kagome materials hosting charge density waves,"The recent discovery of a charge density (CDW) state in ScV$_6$Sn$_6$ at $T_{\textrm{CDW}}$ = 91 K offers new opportunities to understand the origins of electronic instabilities in topological kagome systems. By comparing to the isostructural non-CDW compound LuV$_6$Sn$_6$, we unravel interesting electrical transport properties in ScV$_6$Sn$_6$, above and below the charge ordering temperature. We observed that by applying a magnetic field along the $a$ axis, the temperature behavior of the longitudinal resistivity in ScV$_6$Sn$_6$ changes from metal-like to insulator-like above the CDW transition. We show that in the charge ordered state ScV$_6$Sn$_6$ follows the Fermi liquid behavior while above that, it transforms into a non-Fermi liquid phase in which the resistivity varies sublinearly over a broad temperature range. The sublinear resistivity, which scales by $T^{3/5}$ is a common feature among other vanadium-containing kagome compounds exhibiting CDW states such as KV$_3$Sb$_5$, RbV$_3$Sb$_5$, and CsV$_3$Sb$_5$. By contrast, the non-Fermi liquid behavior does not occur in LuV$_6$Sn$_6$. We explain the $T^{3/5}$ universal scaling behavior from the Coulomb scattering between Dirac electrons and Van Hove singularities; common features in the electronic structure of kagome materials. Finally, we show anomalous Hall-like behavior in ScV$_6$Sn$_6$ below $T_{\textrm{CDW}}$, which is absent in the Lu compound. Comparing the transport properties of ScV$_6$Sn$_6$ and LuV$_6$Sn$_6$ is valuable to highlight the impacts of the unusual CDW in the Sc compound.",2305.02393v2 2014-06-24,The Origin of the X-ray Emission from the High-velocity Cloud MS30.7-81.4-118,"A soft X-ray enhancement has recently been reported toward the high-velocity cloud MS30.7-81.4-118 (MS30.7), a constituent of the Magellanic Stream. In order to investigate the origin of this enhancement, we have analyzed two overlapping XMM-Newton observations of this cloud. We find that the X-ray enhancement is $\sim$6' or $\sim$100 pc across, and is concentrated to the north and west of the densest part of the cloud. We modeled the X-ray enhancement with a variety of spectral models. A single-temperature equilibrium plasma model yields a temperature of $(3.69^{+0.47}_{-0.44}) \times 10^6$ K and a 0.4-2.0 keV luminosity of $7.9 \times 10^{33}$ erg s$^{-1}$. However, this model underpredicts the on-enhancement emission around 1 keV, which may indicate the additional presence of hotter plasma ($T \gtrsim 10^7$ K), or that recombination emission is important. We examined several different physical models for the origin of the X-ray enhancement. We find that turbulent mixing of cold cloud material with hot ambient material, compression or shock heating of a hot ambient medium, and charge exchange reactions between cloud atoms and ions in a hot ambient medium all lead to emission that is too faint. In addition, shock heating in a cool or warm medium leads to emission that is too soft (for reasonable cloud speeds). We find that magnetic reconnection could plausibly power the observed X-ray emission, but resistive magnetohydrodynamical simulations are needed to test this hypothesis. If magnetic reconnection is responsible for the X-ray enhancement, the observed spectral properties could potentially constrain the magnetic field in the vicinity of the Magellanic Stream.",1406.6363v1 2015-03-21,Graphene as a p-type metal for ultimate miniaturization,"We report macroscopic sheets of highly conductive bilayer graphene with exceptionally high hole concentrations of ~ $10^{15}$ $cm^{-2}$ and unprecedented sheet resistances of 20-25 {\Omega} per square over macroscopic scales, and obtained in-situ over a thin cushion of molecular oxygen on a silicon substrate. The electric and electronic properties of this specific configuration remain stable upon thermal anneals and months of exposure to air. We further report a complementary ab-initio study, predicting an enhancement of graphene adhesion energy of up to a factor 20, also supported by experimental fracture tests. Our results show that the remarkable properties of graphene can be realized in a reliable fashion using a high-throughput process. In addition to providing exceptional material properties, the growth process we employed is scalable to large areas so that the outstanding conduction properties of graphene can be harnessed in devices fabricated via conventional semiconductor manufacturing processes. We anticipate that the approach will provide the necessary scalability and reliability for future developments in the graphene nanoscience and technology fields, especially in areas where further miniaturization is hampered by size effects and electrical reliability of classical conductors.",1503.06253v2 2018-04-06,Antisite pairs suppress the thermal conductivity of BAs,"BAs was predicted to have an unusually high thermal conductivity at room temperature of 2000$\,$Wm$^{-1}$$\,$K$^{-1}$, comparable to that of diamond. However, the experimentally measured thermal conductivity of BAs single crystals is an order of magnitude lower. To identify the origin of this large inconsistency, we investigated the lattice structure and potential defects in BAs single crystals at atomic scale using aberration-corrected scanning transmission electron microscopy (STEM). Rather than finding a large concentration As vacancies ($V_\mathrm{As}$), as widely thought to dominate the thermal resistance in BAs crystals, our STEM results showed enhanced intensity of some B columns and reduced intensity of some As columns, suggesting the presence of antisite defects with As$_\mathrm{B}$ (As-atom on B site) and B$_\mathrm{As}$ (B-atom on As site) with significant concentrations. Further calculations show that the antisite pair with As$_\mathrm{B}$ next to B$_\mathrm{As}$ is preferred energetically among the different types of point defects investigated, and confirm that such defects lower the thermal conductivity for BAs. Using a concentration of 6.6$\pm$3$\times$10$^{20}$$\,$cm$^{-3}$ for the antisite pairs estimated from STEM images, thermal conductivity is estimated to be 65-100$\,$Wm$^{-1}$$\,$K$^{-1}$, in reasonable agreement with our measured value. Our study suggests that As$_\mathrm{B}$-B$_\mathrm{As}$ antisite pairs are the primary lattice defects suppressing thermal conductivity of BAs. Possible approaches are proposed for growth of high quality crystals or films with high thermal conductivity.",1804.02381v1 2019-04-08,Characterizations of thermal stability and electrical performance of Au-Ni coating on CuCrZr substrate for high vacuum radio-frequency contact application,"Radio-frequency (RF) contacts-which are an example of electrical contacts-are commonly employed on accelerators and nuclear fusion experimental devices. RF contacts with a current load of 2 kA for steady-state operation were designed for application to the International Thermonuclear Experimental Reactor (ITER) device. In contrast to the typical working conditions of general commercial electrical contacts, those of RF contacts employed on fusion devices include high vacuum, high temperature, and neutron radiation. CuCrZr is currently of interest as a base material for the manufacture of louvers of RF contacts, which has excellent thermal and electrical properties and has low creep rate at 250 {\textdegree}C. In this study, a hard Au coating (Au-Ni) was electroplated on CuCrZr samples and the samples were then subjected to thermal aging treatment at 250 {\textdegree}C for 500 h in order to simulate the vacuum-commissioning process of the ITER. The effects of thermal aging on the hardness, elastic modulus, crystallite size, and compositions of the coating were investigated via microstructural and mechanical characterizations of the coating material. Metal atom migration in different coating layers during thermal aging was characterized and evaluated via scanning electron microscopy/energy dispersive X-ray spectroscopy observations of the cross-sectional surfaces, and the obtained results could be used to directly select the coating thickness for the final RF contact component. The contact resistance-an important parameter of the RF contact-was measured in a dedicated testbed built to simulate fusion reactor conditions between CuCrZr pins and stainless steel plates coated with Au-Ni and Rh, respectively.",1907.07236v1 2020-07-03,Enhanced creep performance in a polycrystalline superalloy driven by atomic-scale phase transformation along planar faults,"Predicting the mechanical failure of parts in service requires understanding their deformation behavior, and associated dynamic microstructural evolution up to the near-atomic scale. Solutes are known to interact with defects generated by plastic deformation, thereby affecting their displacement throughout the microstructure and hence the material mechanical response to solicitation. This effect is studied here in a polycrystalline Ni-based superalloy with two different Nb contents that lead to a significant change in their creep lifetime. Creep testing at 750C and 600 MPa shows that the high-Nb alloy performs better in terms of creep strain rate. Considering the similar initial microstructures, the difference in mechanical behavior is attributed to a phase transformation that occurs along planar faults, controlled by the different types of stacking faults and alloy composition. Electron channeling contrast imaging reveals the presence of stacking faults in both alloys. Microtwinning is observed only in the low-Nb alloy, rationalizing in part the higher creep strain rate. In the high-Nb alloy, atom probe tomography evidences two different types of stacking faults based on their partitioning behavior. Superlattice intrinsic stacking faults (SISF) were found enriched in Nb, Co, Cr and Mo while only Nb and Co was segregated at superlattice extrinsic stacking faults. Based on their composition, a local phase transformation occurring along the faults is suggested, resulting in slower creep strain rate in the high-Nb alloy. In comparison, mainly SISF enriched in Co, Cr, Nb and Mo were found in the low-Nb alloy. Following the results presented here, and those available in the literature, an atomic-scale driven alloy design approach that controls and promotes local phase transformation along planar faults at 750C is proposed, aiming to design superalloys with enhanced creep resistance.",2007.01676v2 2022-03-15,Flexible terahertz photonic light-cage modules for in-core sensing and high temperature applications,"Terahertz (THz) technology is a growing and multi-disciplinary research field, particularly for sensing and telecommunications. A number of THz waveguides have emerged over the past years, which are set to complement the capabilities of existing and bulky free space setups. In most designs however, the guiding region is physically separated from the surroundings, making interactions between light and the environment inefficient. We present photonic THz light cages (THzLCs) operating at THz frequencies, consisting of free-standing dielectric strands, which guide light within a hollow core with immediate access to the environment. We show the versatility and design flexibility of this concept, by 3D-printing several cm-length-scale modules using a single design and four different polymer- and ceramic- materials, which are either rigid, flexible, or resistant to high temperatures. We characterize propagation- and bend-losses for straight- and curved- waveguides, which are of order ~1 dB/cm in the former, and ~2-8 dB/cm in the latter for bend radii below 10 cm, and largely independent of the material. Our transmission experiments are complemented by near-field measurements at the waveguide output, which reveal antiresonant guidance for straight THzLCs, and a deformed fundamental mode in the bent waveguides, in agreement with numerical conformal mapping simulations. We show that these THzLCs can be used either as: (i) flexible, reconfigurable, and bendable modular assemblies; (ii) in-core sensors of structures contained directly inside the hollow core; (iii) high-temperature sensors, with potential applications in industrial monitoring. These THzLCs are a novel and useful addition to the growing library of THz waveguides, marrying the waveguide-like advantages of reconfigurable, diffractionless propagation, with the free-space-like immediacy of direct exposure to the surrounding environment.",2203.08316v1 2022-10-21,Understanding The Reversible Electrodeposition of Al in Low-Cost Room Temperature Molten Salts,"Aluminum is the most earth-abundant metal, is trivalent, is inert in ambient humid air, and has a density approximately four-times that of lithium at room temperature. These attributes make it an attractive material for cost-effective, long-duration storage of electrical energy in batteries. Scientific discoveries in the past decade have established that secondary Al batteries can be created by paring an Al anode with a graphite or transition metal oxide cathode, in imidazolium-based, room-temperature ionic-liquid-Aluminum chloride electrolytes. Here we report findings from a systematic study that sheds light on the structural requirements, physicochemical, and transport properties of the ionic liquid electrolytes responsible for the high reversibility of Al battery anodes. We find that the most important interfacial and transport properties of these electrolytes can be achieved in other electrolytes, including ammonium-based molten salts that are available at costs as much as twenty-times lower than the ionic liquid-Aluminum chloride melt. High Al reversibility in ammonium- and imidazolium-based electrolytes is specifically shown to require a critical ratio of the solvation species, where Lewis acidity and beneficial interfacial reactions continuously etch the alumina resistive interfacial layer and form beneficial solid electrolyte interphase at the anode. We report further that successful development of new electrolyte families that support high Al anode reversibility also provides a good platform for detailed studies of the working mechanisms of an intercalation graphite cathode using X-ray absorption spectroscopy. Our findings therefore open new opportunities for developing simple, cost-effective, room-temperature Al batteries that enable long-duration electrical energy storage.",2210.12131v1 2024-01-18,Spreading of Low-viscosity Ink Filaments Driven by Bath Viscoelasticity in Embedded Printing,"Inks deposited in conventional direct ink writing need to be able to support their own weight and that of the upper layers with minimal deformation to preserve the structural integrity of the three-dimensional (3D) printed parts. This constraint limits the range of usable inks to high-viscosity materials. Embedded printing enables the use of much softer inks by depositing the materials in a bath of another fluid that provides external support, thus diversifying the types of 3D printable structures. The interactions between the ink and bath fluids, however, give rise to a unique type of defect: spreading of the dispensed ink behind the moving nozzle. By printing horizontal threads made of dyed water in baths of Carbopol suspensions, we demonstrate that the spreading can be attributed to the pressure field generated in the viscous bath by the relative motion of the nozzle. As the pressure gradient increases with the viscosity of the bath fluid while the viscosity of the ink resists the flow, a larger bath-to-ink viscosity ratio results in more spreading for low-concentration Carbopol baths. For high-concentration, yield-stress-fluid baths, we find that the steady-state viscosity alone cannot account for the spreading, as the elastic stress becomes comparable to the viscous stress and the bath fluid around the dispensed ink undergoes fluidization and resolidification. By parameterizing the transient rheology of the high-concentration Carbopol suspensions using a simple viscoelastic model, we suggest that the ink spreading is exacerbated by the elasticity but is mitigated by the yield stress as long as the yield stress is low enough to allow steady injection of the ink. These results help illuminate the link between the bath rheology and the printing quality in embedded 3D printing.",2401.09684v1 2001-10-08,"Structural and electronic properties of the Nb$_4$-cluster compound Ga$_{1.33}$Nb$_4$X$_8$ (X = S, Se)","We report resistivity, thermopower and magnetic susceptibility measurements on the Nb$_4$-cluster compounds Ga$_{1.33}$Nb$_4$X$_{8}$ (X = S, Se), derived from vacancy ordered spinels A$_x$T$_4$X$_8$. The cubic selenide phase is insulating and its resistivity crosses over from $\ln{\rho} \sim T^{-1}$ to $\sim T^{-1/2}$ on cooling below 150 K, indicating variable range hopping (VRH) conduction at low temperatures. This is similar to that previously reported for V$_4$ and Mo$_4$ cluster compounds. The rhombohedrally distorted sulfide is metallic and shows a minimum in resistance at $\sim $ 56 K below which the resistivity varies as $\rho(T) \sim T^{-1/2}$. The thermopower of the selenide becomes temperature independent below the crossover temperature. These Nb$_4$ compounds exhibit enhanced Pauli-paramagnetic magnetic susceptibility ($\chi$) irrespective of their transport properties and both undergo a similar transition in $\chi(T) \sim 30$ K. We discuss these properties in the model of hopping conduction under long-range Coulomb repulsion effects and derive consistency between some of the transport and magnetic parameters.",0110155v1 2001-11-06,Spin-dependent electrical transport in ion-beam sputter deposited Fe-Cr multilayers,"The temperature dependence of the electrical resistivity and magnetoresistance of Xe-ion beam sputtered Fe-Cr multilayers has been investigated. The electrical resistivity between 5 and 300 K in the fully ferromagnetic state, obtained by applying a field beyond the saturation field (H_sat) necessary for the antiferromagnetic(AF)-ferromagnetic(FM) field-induced transition, shows evidence of spin-disorder resistivity as in crystalline Fe and an s-d scattering contribution (as in 3d metals and alloys). The sublattice magnetization m(T) in these multilayers has been calculated in terms of the planar and interlayer exchange energies. The additional spin-dependent scattering \Delta \rho (T) = \rho(T,H=0)_AF - \rho(T,H=H_sat)_FM in the AF state over a wide range of temperature is found to be proportional to the sublattice magnetization, both \Delta \rho(T) and m(T) reducing along with the antiferromagnetic fraction. At intermediate fields, the spin-dependent part of the electrical resistivity (\rho_s (T)) fits well to the power law \rho_s (T) = b - cT^\alpha where c is a constant and b and \alpha are functions of H. At low fields \alpha \approx 2 and the intercept b decreases with H much the same way as the decrease of \Delta \rho (T) with T. A phase diagram (T vs. H_sat) is obtained for the field- induced AF to FM transition. Comparisons are made between the present investigation and similar studies using dc magnetron sputtered and molecular beam epitaxy (MBE) grown Fe-Cr multilayers.",0111084v1 2002-10-29,Quantum Resistive Behaviors in the Vortex Liquid Regimes at Finite Temperatures,"Motivated by a {\it mean field-like} resistive behavior in magnetic fields commonly seen in various superconducting (SC) cuprates and organics with strong fluctuation, {\it quantum} SC fluctuation effects on resistive behaviors are reexamined by putting emphasis on their roles in the so-called {\it thermal} vortex liquid regime. By incorporating the quantum fluctuation and a vortex pinning effect in the GL fluctuation theory, it is found that the resistivity curve shows not a fan-shaped broadening but a sharp drop at a 3d vortex-glass transition point far below an apparent upper critical field H_{c2}^*(T) as a result of a quantm fluctuation enhanced by an adequately small condensation energy or by a strong field. Fittings to data of cuprate and organic superconductors are performed by including effects of SC pseudogap region. It is argued on the cuprate materials that, irrespective of the presence of fluctuations of competing non-SC orders, the in-plane coherence length of hole-doped cuprates decreases on approaching the underdoped limit and that the condensation energy density to be measured from the heat capacity data is maximum near the optimal doping. The case of disordered quasi 2d s-wave films showing the field-tuned superconductor-insulator transition (FSIT) behavior is also studied for comparison, and an agreement with available data is found.",0210626v5 2002-11-22,Room Temperature Ballistic Conduction in Carbon Nanotubes,"Multiwalled carbon nanotubes are shown to be ballistic conductors at room temperature, with mean free paths of the order of tens of microns. These experiments follow and extend the original experiments by Frank et al (Science, 280 1744 1998) including in-situ electron microscopy experiments and a detailed analysis of the length dependence of the resistance. The per unit length resistance r < 100 Ohm/micron, indicating free paths l > 65 microns, unambiguously demonstrate ballistic conduction at room temperature up to macroscopic distances. The nanotube-metal contact resistances are in the range 0.1-1 kOhm micron. Contact scattering can explain why the measured conductances are about half the expected theoretical value of 2 G0 . For V>0.1V the conductance rises linearly (dG/dV~0.3 G0 /V) reflecting the linear increase in the density-of-states in a metallic nanotube above the energy gap. Increased resistances (r =2- 10 k Ohm/micron) and anomalous I-V dependences result from impurities and surfactants on the tubes.Evidence is presented that ballistic transport occurs in undoped and undamaged tubed for which the top layer is metallic and the next layer is semiconducting. The diffusive properties of lithographically contacted multiwalled nanotubes most likely result from purification and other processing steps that damage and dope the nanotubes thereby making them structurally and electronically different than the pristine nanotubes investigated here.",0211515v1 2006-12-27,"Peculiarities of the transport properties of InMnAs layers, produced by the laser deposition, in strong magnetic fields","Magnetotransport properties of p-InMnAs layers are studied in pulsed magnetic fields up to 30 T. Samples were prepared by the laser deposition and annealed by ruby laser pulses. Well annealed samples show p-type conductivity while they were n-type before the annealing. Surprisingly the anomalous Hall effect resistance in paramagnetic state (T>40 K) and in strong magnetic fields (B > 20 T) appears to be greater than that in ferromagnetic state (T <= 40 K), while the longitudinal resistance rises with the temperature decrease. The negative magnetoresistance saturates in magnetic fields higher then 10T at T near 4 K only, whereas the saturation fields of the anomalous Hall effect resistance are much less (around 2 T at 30K). The total reduction of resistance exceeds 10 times in magnetic fields around of 10T. The obtained results are interpreted on the base of the assumptions of the non-uniform distribution of Mn atoms acting as acceptors, the local ferromagnetic transition and the percolation-like character of the film conductivity, which prevailed under conditions of the strong fluctuations of the exchange interaction. Characteristic scales of the magneto-electric nonuniformity are estimated using analysis of the mesoscopic fluctuations of the non-diagonal components of the magnetoresistivity tensor.",0612641v1 2007-06-28,Emergence of a flux tube through a partially ionised solar atmosphere,"For a magnetic flux tube, or indeed any flux, to emerge into the Solar corona from the convection zone it must pass through the partially ionised layers of the lower atmosphere: the photosphere and the chromosphere. In such regions the ion-neutral collisions lead to an increased resistivity for currents flowing across magnetic field lines. This Cowling resistivity can exceed the Spitzer resistivity by orders of magnitude and in 2.5D simulations has been shown to be sufficient to remove all cross field current from emerging flux. Here we extend this modelling into 3D. Once again it is found that the Cowling resistivity removes perpendicular current. However the presence of 3D structure prevents the simple comparison possible in 2.5D simulations. With a fully ionised atmosphere the flux emergence leads to an unphysically low temperature region in the overlying corona, lifting of chromospheric material and the subsequent onset of the Rayleigh-Taylor instability. Including neutrals removes the low temperature region, lifts less chromospheric matter and shows no signs of the Rayleigh-Taylor instability. Simulations of flux emergence therefore should include such a neutral layer in order to obtain the correct perpendicular current, remove the Rayleigh-Taylor instability and get the correct temperature profile. In situations when the temperature is not important, i.e. when no simulated spectral emission is required, a simple model for the neutral layer is demonstrated to adequately reproduce the results of fully consistent simulations.",0706.4223v1 2010-01-10,Anomalies of conductivity behavior near the paramagnetic-antiferromagnetic transition in single-crystals La_{2}CuO_{4+δ},"The temperature dependences of resistance, R(T), of two single-crystals La_{2}CuO_{4+\delta} samples have been studied with the aim to detect a possible change in the R(T) behavior induced by paramagnetic-antiferromagnetic (PM-AFM) transition. One of the samples with \delta \lesssim 0.01, was fairly homogeneous in oxygen distribution (not phase-separated) with Neel temperature T_{N}\approx 266 K. Conductivity of this sample has been determined by Mott's variable-range hopping below T_N. The other, far less resistive, sample with \delta \approx 0.05, was inhomogeneous (phase-separated) showing both PM-AFM (T_N\approx 205 K) and superconducting (T_c\approx 25 K) transitions. It is found that for the homogeneous sample the resistivity decreases above T_N far faster with temperature than below it (for both directions of measuring current, parallel and perpendicular to basal CuO_2 planes). A similar behavior of conductivity near PM-AFM transition is also found for the phase-separated and less resistive sample. In this case a clear kink in R(T) curve near T_N\approx 205 K can be seen. Furthermore, a transition to metallic (dR/dT>0) behavior occurs far enough above T_N. The observed behavior of the samples studied is related to increased delocalization of charge carriers above T_N. This is in accordance with decrease in the AFM correlation length and corresponding enhancement of the hole mobility above T_N known for low-doped lanthanum cuprates.",1001.1518v1 2011-05-07,Effect of 50 MeV Li3+ irradiation on structural and electrical properties of Mn doped ZnO,"The present work aims to study the effect of ion irradiation on structural and electrical properties and their correlation with the defects in Zn1-xMnxO type system. Zn1-xMnxO (x = 0.02, 0.04) samples have been synthesized by solid-state reaction method and have been irradiated with 50 MeV Li3+ ions. The concomitant changes have been probed by x-ray diffraction (XRD), temperature dependent electrical resistivity and positron annihilation lifetime (PAL) spectroscopy. XRD result shows single phase wurtzite structure for Zn0.98Mn0.02O, whereas for Zn0.96Mn0.04O sample an impurity phase has been found apart from the usual peaks of ZnO. Ion irradiation dissolves this impurity peak. Grain size of the samples found to be uniform. For Zn0.98Mn0.02O, the observed sharp decrease in room temperature resistivity (RhoRT) with irradiation is consistent with the lowering of FWHM of the XRD peaks. However for Zn0.96Mn0.04O, RhoRT decreases for initial fluence but increases for further increase of fluence. All the irradiated Zn0.98Mn0.02O samples show metal-semiconductor transition in temperature dependent resistivity measurement at low temperature. But all the irradiated Zn0.96Mn0.04O samples show semiconducting nature in the whole range of temperature. Results of room temperature resistivity, XRD and PAL measurements are consistent with each other.",1105.1414v1 2013-01-07,Disorder-driven carrier transport in atomic layer deposited ZnO thin films,"This paper addresses the effect of disorder on the carrier transport mechanism of atomic layer deposited ZnO thin films as has been investigated by temperature dependent electrical resistivity measurements in the temperature range of 4.2K to 300K. Films were grown on (0001) sapphire substrate at different substrate temperatures varying from 150 to 350 C. The defects and structural disorder in the films were found to be strongly dependent on their growth temperature. The films grown at 150, 300 and 350 C were found to be semiconductor-like in the whole measurement temperature range of resistivity due to the enhanced disorder in these films. However, a metal to semiconductor transition (MST) at low temperature has been observed in the films grown at 200 and 250 C. It was also observed that the film grown at 250 C with higher residual resistivity, the transition temperature shifted towards the higher value due to the increased disorder in this film as compared to that grown at 200 C. The upturn in resistivity below the transition temperature has been well explained by considering quantum corrections to the Boltzmanns conductivity which includes the effect of weak localization and coulomb electron-electron interactions related to the existence of disorder in these films.",1301.1172v1 2014-11-27,Temperature dependence of electrical and thermal conduction in single silver nanowire,"Silver nanowires have great application potential in fields like flexible electronic devices, solar cells and transparent electrodes. It is critical and fundamental to study the thermal and electrical transport properties in a single silver nanowire. In this work, the thermal and electrical transport in an individual silver nanowire is characterized down to 35 K with the steady state electro-thermal technique. The results indicate that, at room temperature, the electrical resistivity increases by around 4 folds compared from that of its bulk counterpart. After fitting the temperature dependent electrical resistivity curves with the Bloch-Gr\""uneisen formula, the Debye temperature (151 K) of the silver nanowire is found 36% lower than that (235 K) of bulk silver, confirming strong phonon softening. The thermal conductivity is reduced by 55% compared with that of its bulk counterpart at room temperature and this reduction becomes larger as the temperature goes down. To explain the opposite trends of thermal conductivity (\k{appa}) ~ temperature (T) of silver nanowire and bulk silver, a unified thermal resistivity is used to elucidate the electron scattering mechanism. A large residual unified thermal resistivity for the silver nanowire is observed while that of the bulk silver is almost zero. The same trend of variation against T indicates that the silver nanowire and bulk silver share the same phonon-electron scattering mechanism. Additionally, due to phonon-assisted electron energy transfer across the grain boundaries, the Lorenz number of the silver nanowire is found much larger than that of bulk silver and decreases with decreasing temperature.",1411.7659v2 2015-09-18,Evidence for hydrodynamic electron flow in PdCoO$_2$,"Electron transport is conventionally determined by the momentum-relaxing scattering of electrons by the host solid and its excitations. The electrical resistance is set by geometrical factors and the resistivity, which is a microscopic property of the solid. Hydrodynamic fluid flow through channels, in contrast, is determined by geometrical factors, boundary scattering and the viscosity of the fluid, which is governed by momentum-conserving internal collisions. A long-standing question in the physics of solids, brought into focus by the advent of new calculational techniques, has been whether the viscosity of the electron fluid plays an observable role in determining the resistance. At first sight this seems unlikely, because in almost all known materials the rate of momentum-relaxing collisions dominates that of the momentum-conserving ones that give the viscous term. Here, we show this is not always the case. We report experimental evidence that the resistance of restricted channels of the ultra-pure two-dimensional metal PdCoO$_2$ has a large viscous contribution. Comparison with theory allows an estimate of the electronic viscosity in the range between $6\times 10^{-3}$~kg(ms)$^{-1}$ and $3\times 10^{-4}$~kg(ms)$^{-1}$, which brackets that of water at room temperature.",1509.05691v2 2015-10-31,The influence of system dynamics on the frictional resistance: insights from a discrete model,"In order to examine the influence of system dynamics on sliding friction, we introduce the so-called micro-walking machine. This model consists of a rigid body with a number of elastic contact spots that is pulled by a constantly moving base. The system slides with dry friction on a rigid substrate. The kinematic coupling of the rotation and the translation of the rigid body results in varying normal and tangential forces at the contact spots. For certain parameter ranges this leads to self-excited oscillations in the vertical direction. A particular dynamic mode occurs which is characterized by a strong correlation between low or even zero normal forces and a fast forward motion. This effect is referred to as micro-walking. In addition to an experimental rig we use numerical integration and an extensive parameter study for the analysis. In theory, the reduction of the frictional resistance reaches up to 98%. These results are confirmed by the experiments where the maximal reduction was 73%. Our model shows that micro-vibrations play an important role for the dynamic influences on the frictional resistance of systems that exhibit apparently smooth sliding. The identification of the critical parameter range enables the systematic control of frictional resistance through the adjustment of attributes such as geometry and stiffness. In addition, it is possible to deduce guidelines for how tribological test rigs should be designed in order to get reliable results.",1511.00162v1 2016-05-02,Interfilament Resistance at 77 K in Striated HTS Coated Conductors,"Striating HTS coated conductor (CC) tapes into narrow filaments offers the possibility of reducing the tapes' magnetization losses without unreasonably decreasing their current-carrying capability. However, realizing well-separated striations presents technological challenges, especially if the number of filaments is large and/or if a thick layer of metallic stabilizer is present. In these situations, the filaments can be easily coupled and their effectiveness to reduce magnetization losses is strongly diminished or eliminated. While the onset of coupling is well visible from magnetization loss measurements, the actual path of the coupling current is unknown. In this contribution we present a systematic study of the transverse resistance in HTS CC samples in order to get a deeper understanding of those paths. The measured samples differ in terms of manufacturer (SuperPower and SuperOx), and presence and thickness of stabilizer material. In addition, oxidation is used as a means to increase the resistance between the filaments in non-stabilized samples. The results are interpreted with a chain network model. This work provides useful insights on the factors determining the transverse resistance in striated HTS CCs, thus indicating ways to improve the effectiveness of the striation process for AC loss reduction.",1605.00401v2 2016-08-09,Disorder-sensitive pump-probe measurements on Nd$_{1.83}$Ce$_{0.17}$CuO$_{4\pmδ}$ films,"We find an unambiguous relationship between disorder-driven features in the temperature dependence of the resistance and the behavior, as functions of the temperature, of the parameters necessary to describe some of the relaxation processes in the photoinduced differential time-resolved reflectivity of three samples of Nd$_{1.83}$Ce$_{0.17}$CuO$_{4\pm\delta}$. The latter, sharing the same Ce content, have been fabricated and annealed ad-hoc in order to differ only for the degree of disorder, mainly related to oxygen content and location, and, consequently, for the temperature dependence of the resistance: two of them present a minimum in the resistance and behave as a superconductor and as a metal, respectively, the third behaves as an insulator. The systematic coherence between the resistance and the relaxation parameters behaviors in temperature for all three samples is absolutely remarkable and shows that pump-probe measurements can be extremely sensitive to disorder as it drives the emergence of new excitations and of the related relaxation channels as in this paradigmatic case.",1608.03006v1 2018-05-10,Activation Energy of Metastable Amorphous Ge2Sb2Te5 from Room Temperature to Melt,"Resistivity of metastable amorphous Ge2Sb2Te5 (GST) measured at device level show an exponential decline with temperature matching with the steady-state thin-film resistivity measured at 858 K (melting temperature). This suggests that the free carrier activation mechanisms form a continuum in a large temperature scale (300 K - 858 K) and the metastable amorphous phase can be treated as a super-cooled liquid. The effective activation energy calculated using the resistivity versus temperature data follow a parabolic behavior, with a room temperature value of 333 meV, peaking to ~377 meV at ~465 K and reaching zero at ~930 K, using a reference activation energy of 111 meV (3kBT/2) at melt. Amorphous GST is expected to behave as a p-type semiconductor at Tmelt ~ 858 K and transitions from the semiconducting-liquid phase to the metallic-liquid phase at ~ 930 K at equilibrium. The simultaneous Seebeck (S) and resistivity versus temperature measurements of amorphous-fcc mixed-phase GST thin-films show linear S-T trends that meet S = 0 at 0 K, consistent with degenerate semiconductors, and the dS/dT and room temperature activation energy show a linear correlation. The single-crystal fcc is calculated to have dS/dT = 0.153 {\mu}V/K for an activation energy of zero and a Fermi level 0.16 eV below the valance band edge.",1805.04054v1 2019-09-17,Algorithm for Training Neural Networks on Resistive Device Arrays,"Hardware architectures composed of resistive cross-point device arrays can provide significant power and speed benefits for deep neural network training workloads using stochastic gradient descent (SGD) and backpropagation (BP) algorithm. The training accuracy on this imminent analog hardware however strongly depends on the switching characteristics of the cross-point elements. One of the key requirements is that these resistive devices must change conductance in a symmetrical fashion when subjected to positive or negative pulse stimuli. Here, we present a new training algorithm, so-called the ""Tiki-Taka"" algorithm, that eliminates this stringent symmetry requirement. We show that device asymmetry introduces an unintentional implicit cost term into the SGD algorithm, whereas in the ""Tiki-Taka"" algorithm a coupled dynamical system simultaneously minimizes the original objective function of the neural network and the unintentional cost term due to device asymmetry in a self-consistent fashion. We tested the validity of this new algorithm on a range of network architectures such as fully connected, convolutional and LSTM networks. Simulation results on these various networks show that whatever accuracy is achieved using the conventional SGD algorithm with symmetric (ideal) device switching characteristics the same accuracy is also achieved using the ""Tiki-Taka"" algorithm with non-symmetric (non-ideal) device switching characteristics. Moreover, all the operations performed on the arrays are still parallel and therefore the implementation cost of this new algorithm on array architectures is minimal; and it maintains the aforementioned power and speed benefits. These algorithmic improvements are crucial to relax the material specification and to realize technologically viable resistive crossbar arrays that outperform digital accelerators for similar training tasks.",1909.07908v1 2017-04-13,Light Induced Electron-Phonon Scattering Mediated Resistive Switching in Nanostructured Nb Thin Film Superconductor,"The elemental Nb is mainly investigated for its eminent superconducting properties. In contrary, we report of a relatively unexplored property, namely, its superior optoelectronic property in reduced dimension. We demonstrate here that nanostructured Nb thin films (NNFs), under optical illumination, behave as room temperature photo-switches and exhibit bolometric features below its superconducting critical temperature. Both photo-switch and superconducting bolometric behavior are monitored by its resistance change with light in visible and near infrared (NIR) wavelength range. Unlike the conventional photodetectors, the NNF devices switch to higher resistive states with light and the corresponding resistivity change is studied with thickness and grain size variations. At low temperature in its superconducting state, the light exposure shifts the superconducting transition towards lower temperature. The room temperature photon sensing nature of the NNF is explained by the photon assisted electron-phonon scattering mechanism while the low temperature light response is mainly related to the heat generation which essentially changes the effective temperature for the device and the device is capable of sensing a temperature difference of few tens of milli-kelvins. The observed photo-response on the transport properties of NNFs can be very important for future superconducting photon detectors, bolometers and phase slip based device applications.",1704.04092v1 2017-07-05,Anomalous Hall effect in two-dimensional non-collinear antiferromagnetic semiconductor Cr0.68Se,"Cr0.68Se single crystals with two-dimensional (2D) character have been grown, and the detailed magnetization M(T), electrical transport properties (including longitudinal resistivity and Hall resistivity and thermal transport ones (including heat capacity Cp(T) and thermoelectric power (TEP) S(T)) have been measured. There are some interesting phenomena: (i) Cr0.68Se presents a non-collinear antiferromagnetic (AFM) semiconducting behavior with the Neel temperature TN = 42 K and the activated energy Eg=3.9 meV; (ii) It exhibits the anomalous Hall effect (AHE) below TN and large negative magnetoresistance (MR) about 83.7% (2 K, 8.5 T). The AHE coefficient RS is 0.385 cm-3/C at T=2 K and the AHE conductivity {\sigma}H is about 1 ohm-1cm-1 at T=40 K, respectively; (iii) The scaling behavior between the anomalous Hall resistivity and the longitudinal resistivity is linear and further analysis implies that the origin of the AHE in Cr0.68Se is dominated by the skew-scattering mechanism. Our results may be helpful for exploring the potential application of these kind of 2D AFM semiconductors.",1707.01252v1 2017-07-20,Stochastic Dynamics of Resistive Switching: Fluctuations Lead to Optimal Particle Number,"Resistive switching is one of the foremost candidates for building novel types of non-volatile random access memories. Any practical implementation of such a memory cell calls for a strong miniaturization, at which point fluctuations start playing a role that cannot be neglected. A detailed understanding of switching mechanisms and reliability is essential. For this reason, we formulate a particle model based on the stochastic motion of oxygen vacancies. It allows us to investigate fluctuations in the resistance states of a switch with two active zones. The vacancies' dynamics is governed by a master equation. Upon the application of a voltage pulse, the vacancies travel collectively through the switch. By deriving a generalized Burgers equation we can interpret this collective motion as nonlinear traveling waves, and numerically verify this result. Further, we define binary logical states by means of the underlying vacancy distributions, and establish a framework of writing and reading such memory element with voltage pulses. Considerations about the dis- criminability of these operations under fluctuations together with the markedness of the resistive switching effect itself lead to the conclusion, that an intermediate vacancy number is optimal for performance.",1707.06648v1 2018-08-02,Non-Classical Longitudinal Magneto-Resistance in Anisotropic Black Phosphorus,"Resistivity measurements of a few-layer black phosphorus (bP) crystal in parallel magnetic fields up to 45 T are reported as a function of the angle between the in-plane field and the source-drain (S-D) axis of the device. The crystallographic directions of the bP crystal were determined by Raman spectroscopy, with the zigzag axis found within 5{\deg} of the S-D axis, and the armchair axis in the orthogonal planar direction. A transverse magneto-resistance (TMR) as well as a classically-forbidden longitudinal magneto-resistance (LMR) are observed. Both are found to be strongly anisotropic and non-monotonic with increasing in-plane field. Surprisingly, the relative magnitude (in %) of the positive LMR is larger than the TMR above $\sim$32 T. Considering the known anisotropy of bP whose zigzag and armchair effective masses differ by a factor of approximately seven, our experiment strongly suggests this LMR to be a consequence of the anisotropic Fermi surface of bP.",1808.00858v2 2019-08-12,The role of graphitic filaments in resistive switching behaviour of amorphous silicon carbide thin films,"Resistive switching in amorphous silicon carbide (a-SiC) films deposited by a single composite target magnetron sputtering process is reported. Switching performance as a function of thickness of the films (50, 100 and 300 nm) as well as different top metal electrodes (Cu, Pt and Ag) with the bottom electrode fixed as Au, is investigated. The switching parameters (Forming Voltage, Set and Reset voltages and corresponding currents) are found to be dependent on thickness of SiC films and it is observed that 100 nm is the optimal thickness for best endurance. The interface between metal electrode and a-SiC films plays a more significant role in achieving switching performance. Resistance Off/On ratios of 108, retention times >104 s and endurance of 50 cycles are achieved in the best devices. Cross-sectional scanning electron microscopy provides evidence that the mechanism of switching involves the formation of carbonaceous filaments and Raman spectroscopy indicates that these filaments are nanocrystalline graphite in nature. The current work clearly establishes that there is dissociation of SiC during the switching cycles leading to formation of nanocrystalline graphitic filaments. These contribute to switching, in addition to the metallic filaments, in the a-SiC based resistive memory device.",1908.04079v1 2018-07-13,Tuning vortex fluctuations and the resistive transition in superconducting films with a thin overlayer,"It is shown that the temperature of the resistive transition $T_r$ of a superconducting film can be increased by a thin superconducting or normal overlayer. For instance, deposition of a highly conductive thin overlayer onto a dirty superconducting film can give rise to an ""anti-proximity effect"" which manifests itself in an initial increase of $T_r(d_2)$ with the overlayer thickness $d_2$ followed by a decrease of $T_r(d_2)$ at larger $d_2$. Such a nonmonotonic thickness dependence of $T_r(d_2)$ results from the interplay of the increase of a net superfluid density mitigating phase fluctuations and the suppression of the critical temperature $T_c$ due to the conventional proximity effect. This behavior of $T_r(d_2)$ is obtained by solving the Usadel equations to calculate the temperature of the Berezinskii-Kosterletz-Thouless transition, and the temperature of the resistive transition due to thermally-activated hopping of single vortices in dirty bilayers. The theory incorporates relevant materials parameters such as thicknesses and conductivities of the layers, interface contact resistance between them and the subgap quasiparticle states which affect both phase fluctuations and the proximity effect suppression of $T_c$. The transition temperature $T_r$ can be optimized by tuning the overlayer parameters, which can significantly weaken vortex fluctuations and nearly restore the mean-field critical temperature. The calculated behavior of $T_r(d_2)$ may explain the nonmonotonic dependence of $T_r(d_2)$ observed on (Ag, Au, Mg, Zn)-coated Bi films, Ag-coated Ga and Pb films or NbN and NbTiN films on AlN buffer layers. These results suggest that bilayers can be used as model systems for systematic investigations of optimization of fluctuations in superconductors.",1807.04891v1 2020-01-02,Numerical investigation into fracture resistance of bone following adaptation,"Bone adapts in response to its mechanical environment. This evolution of bone density is one of the most important mechanisms for developing fracture resistance. A finite element framework for simulating bone adaptation, commonly called bone remodelling, is presented. This is followed by a novel method to both quantify fracture resistance and to simulate fracture propagation. The authors' previous work on the application of configurational mechanics for modelling fracture is extended to include the influence of heterogeneous bone density distribution. The main advantage of this approach is that configurational forces, and fracture energy release rate, are expressed exclusively in terms of nodal quantities. This approach avoids the need for post-processing and enables a fully implicit formulation for modelling the evolving crack front. In this paper density fields are generated from both (a) bone adaptation analysis and (b) subject-specific geometry and material properties obtained from CT scans. It is shown that, in order to correctly evaluate the configurational forces at the crack front, it is necessary to have a spatially smooth density field with higher regularity than if the field is directly approximated on the finite element mesh. Therefore, discrete density data is approximated as a smooth density field using a Moving Weighted Least Squares method. Performance of the framework is demonstrated using numerical simulations for bone adaptation and subsequent crack propagation, including consideration of an equine 3rd metacarpal bone. The degree of bone adaption is shown to influence both fracture resistance and the resulting crack path.",2001.00647v1 2020-06-19,Contrasting physical properties of the trilayer nickelates Nd$_4$Ni$_3$O$_{10}$ and Nd$_4$Ni$_3$O$_8$,"We report the crystal structures and physical properties of trilayer nickelates Nd$_4$Ni$_3$O$_{10}$ and Nd$_4$Ni$_3$O$_8$. Measurements of magnetization and electrical resistivity display contrasting behaviors in the two compounds. Nd$_4$Ni$_3$O$_{10}$ shows a paramagnetic metallic behavior with a metal to metal phase transition($T^{\ast}$) at about 162 K, as revealed by both magnetic susceptibility and resistivity. Further magnetoresistance and Hall coefficient results show a negative magnetoresistance at low temperatures and the carrier type of Nd$_4$Ni$_3$O$_{10}$ is dominated by hole-type charge carriers. The significant enhancement of Hall coefficient and resistivity below $T^{\ast}$ suggest that effective charge carrier density decreases when cooling through the transition temperature. In contrast, Nd$_4$Ni$_3$O$_8$ shows an insulating behavior despite small value of resistivity at room temperature. The compound shows paramagnetic behavior, with the similar magnetic moments as in Nd$_4$Ni$_3$O$_{10}$ derived from the Curie-Weiss fitting. This may suggest that the magnetic moments in both systems are contributed by the Nd ions. By applying pressures up to about 49 GPa, the insulating behavior is still present and becomes even stronger. Our results suggest that the different Ni configurations ($Ni^{1+/2+}$ or $Ni^{2+/3+}$) and competition between localized and itinerant electrons may account for the contrasting behaviors in trilayer nickelates Nd$_4$Ni$_3$O$_{10}$ and Nd$_4$Ni$_3$O$_8$.",2006.10988v1 2020-10-13,How to solve problems in micro- and nanofabrication caused by the emission of electrons and charged metal atoms during e-beam evaporation,"We discuss how the emission of electrons and ions during electron-beam-induced physical vapor deposition can cause problems in micro- and nanofabrication processes. After giving a short overview of different types of radiation emitted from an electron-beam (e-beam) evaporator and how the amount of radiation depends on different deposition parameters and conditions, we highlight two phenomena in more detail: First, we discuss an unintentional shadow evaporation beneath the undercut of a resist layer caused by the one part of the metal vapor which got ionized by electron-impact ionization. These ions first lead to an unintentional build-up of charges on the sample, which in turn results in an electrostatic deflection of subsequently incoming ionized metal atoms towards the undercut of the resist. Second, we show how low-energy secondary electrons during the metallization process can cause cross-linking, blisters, and bubbles in the respective resist layer used for defining micro- and nanostructures in an e-beam lithography process. After the metal deposition, the cross-linked resist may lead to significant problems in the lift-off process and causes leftover residues on the device. We provide a troubleshooting guide on how to minimize these effects, which e.g. includes the correct alignment of the e-beam, the avoidance of contaminations in the crucible and, most importantly, the installation of deflector electrodes within the evaporation chamber.",2010.06459v2 2021-02-17,Optimization of epitaxial graphene growth for quantum metrology,"(See the complete abstract within the thesis in both English and German versions) In this thesis, the process conditions of the epitaxial graphene growth through a socalled polymer-assisted sublimation growth method are minutely investigated. Atomic force microscopy (AFM) is used to show that the previously neglected flow-rate of the argon process gas has a significant influence on the morphology of the SiC substrate and atop carbon layers. The results can be well explained using a simple model for the thermodynamic conditions at the layer adjacent to the surface. The resulting control option of step-bunching on the sub-nanometer scales is used to produce the ultra-flat, monolayer graphene layers without the bilayer inclusions that exhibit the vanishing of the resistance anisotropy. The comparison of four-point and scanning tunneling potentiometry measurements shows that the remaining small anisotropy represents the ultimate limit, which is given solely by the remaining resistances at the SiC terrace steps. ... The precise control of step-bunching using the Ar flow also enables the preparation of periodic non-identical SiC surfaces under the graphene layer. Based on the work function measurements by Kelvin-Probe force microscopy and X-ray photoemission electron microscopy, it is shown for the first time that there is a doping variation in graphene, induced by a proximity effect of the different near-surface SiC stacks. The comparison of the AFM and low-energy electron microscopy measurements have enabled the exact assignment of the SiC stacks, and the examinations have led to an improved understanding of the surface restructuring in the framework of a step-flow mode. ...",2102.08691v1 2021-05-30,Enhanced electron-phonon coupling in doubly aligned hexagonal boron nitride bilayer graphene heterostructure,"The relative twist angle in heterostructures of two-dimensional (2D) materials with similar lattice constants result in a dramatic alteration of the electronic properties. Here, we investigate the electrical and magnetotransport properties in bilayer graphene (BLG) encapsulated between two hexagonal boron nitride (hBN) crystals, where the top and bottom hBN are rotationally aligned with bilayer graphene with a twist angle $\theta_t\sim 0^{\circ} \text{and}~ \theta_b < 1^{\circ}$, respectively. This results in the formation of two moir\'e superlattices, with the appearance of satellite resistivity peaks at carrier densities $n_{s1}$ and $n_{s2}$, in both hole and electron doped regions, together with the resistivity peak at zero carrier density. Furthermore, we measure the temperature(T) dependence of the resistivity ($\rho$). The resistivity shows a linear increment with temperature within the range 10K to 50K for the density regime $n_{s1} 10^3$) than control devices ($<10^2$), and a median set voltage lower by approximately 1 V (~35%), with a corresponding reduction of the switching power. Our $HfO_x+GST$ RRAM shows 2x gradual switching range using fast (~ns) identical pulse trains with amplitude less than 2 V.",2203.12190v1 2022-05-09,Reconciling scaling of the optical conductivity of cuprate superconductors with Planckian resistivity and specific heat,"Materials tuned to a quantum critical point display universal scaling properties as a function of temperature $T$ and frequency $\omega$. A long-standing puzzle regarding cuprate superconductors has been the observed power-law dependence of optical conductivity with an exponent smaller than one, in contrast to $T$-linear dependence of the resistivity and $\omega$-linear dependence of the optical scattering rate. Here, we present and analyze resistivity and optical conductivity of La$_{2-x}$Sr$_x$CuO$_4$ with $x=0.24$. We demonstrate $\hbar\omega/k_{\mathrm{B}} T$ scaling of the optical data over a wide range of frequency and temperature, $T$-linear resistivity, and optical effective mass proportional to $\sim \ln T$ corroborating previous specific heat experiments. We show that a $T,\omega$-linear scaling Ansatz for the inelastic scattering rate leads to a unified theoretical description of the experimental data, including the power-law of the optical conductivity. This theoretical framework provides new opportunities for describing the unique properties of quantum critical matter.",2205.04030v2 2022-05-23,Electrical Resistivity of Polycrystalline Graphene: Effect of Grain-Boundary-Induced Strain Fields,"We have revealed the decisive role of grain-boundary-induced strain fields in electron scattering in polycrystalline graphene. To this end, we have formulated the model based on Boltzmann transport theory which properly takes into account the microscopic structure of grain boundaries (GB) as a repeated sequence of heptagon-pentagon pairs. The effect of strain field is described within the deformation potential theory. For comparison, we consider the scattering due to electrostatic potential of charged grain boundary. We show that at naturally low GB charges the deformation potential scattering dominates and leads to physically reasonable and, what is important, experimentally observable values of the electrical resistivity. It ranges from 0.1 to 10 k$\Omega $$\mu $m for different types of GBs with a size of 1 $\mu$m and has a strong dependence on misorientation angle. For low-angle highly charged GBs, two scattering mechanisms may compete. The resistivity increases markedly with decreasing GB size and reaches values of 60 k$\Omega $$\mu $m and more. It is also very sensitive to the presence of irregularities modeled by embedding of partial disclination dipoles. With significant distortion, we found an increase in resistance by more than an order of magnitude, which is directly related to the destruction of diffraction on the GB. Our findings may be of interest both in the interpretation of experimental data and in the design of electronic devices based on poly- and nanocrystalline graphene.",2205.11270v1 2022-05-31,Anisotropic signatures of the electronic correlations in the electrical resistivity of UTe$_2$,"Multiple unconventional superconducting phases are suspected to be driven by magnetic fluctuations in the heavy-fermion paramagnet UTe$_2$, and a challenge is to identify the signatures of the electronic correlations, including the magnetic fluctuations, in the bulk physical quantities. Here, we investigate thoroughly the anisotropy of the electrical resistivity of UTe$_2$ under intense magnetic fields up to 70~T, for different electrical-current and magnetic-field configurations. Two characteristic temperatures and an anisotropic low-temperature Fermi-liquid-like coefficient $A$, controlled by the electronic correlations, are extracted. Their critical behavior near the metamagnetic transition induced at $\mu_0H_m\simeq35$~T for $\mathbf{H}\parallel\mathbf{b}$ is characterized. Anisotropic scattering processes are evidenced and magnetic fluctuations are proposed to contribute, via a Kondo hybridization, to the electrical resistivity. Our work appeals for a microscopic modeling of the anisotropic contributions to the electrical resistivity as a milestone for understanding magnetically-mediated superconductivity in UTe$_2$.",2205.15789v2 2022-06-11,"On the Fermi gas, the Sommerfeld fine structure constant, and the electron-electron scattering in conductors","Electrical energy is considered as a fundamental parameter for inclusion in Fermi gas theory, in addition to thermal energy. It is argued that electrical energy can move some electrons to above the Fermi Level, providing free charges to carry the electrical current, even at absolute zero temperature. The Drude model, Ohm's law, quantum resistance, and the electrical resistivity due to electron-electron scattering appear naturally as a consequence of the theoretical description, which is based on the quantization of the angular momentum and the Fermi-Dirac distribution, considering total energy as ${\epsilon}$ = k$_B$$T$ + ${\Phi}_0$$I$. The electrical and magnetic forces acting on an electron are related to the ratio between the Fermi velocity and the speed of light and show that the electron motion is due to helical paths. Considering the center of mass description for the Bohr atom, it was possible to show that the magnetic force is related to the electrical force as $F_M$ = (${\alpha}$/${\pi}$) $F_E$, which demonstrates that the electrons move in helical paths along the orbit. The helical motion naturally provides for quantization of the magnetic flux, the spin of the electron, and the first correction term of the anomalous magnetic moment. Applying the model to describe the electron-electron scattering allows prediction of the behavior of the electrical resistivity of many metals at low temperatures, which is in excellent agreement with empirical observations.",2206.05393v2 2022-06-30,Antipolar transitions in GaNb$_4$Se$_8$ and GaTa$_4$Se$_8$,"We present dielectric, polarization, resistivity, specific heat, and magnetic susceptibility data on single crystals of the lacunar spinels GaNb4Se8 and GaTa4Se8, tetrahedral cluster-based materials with substantial spin-orbit coupling. We concentrate on the possible occurrence of antipolar order in these compounds, as previously reported for the isoelectronic GaNb4S8, where spin-orbit coupling plays a less important role. Our broadband dielectric-spectroscopy investigations reveal clear anomalies of the intrinsic dielectric constant at the magneto-structural transitions in both systems that are in accord with the expectations for antipolar transitions. A similar anomaly is also observed at the cubic-cubic transition of the Nb compound leading to an intermediate phase. Similar to other polar and antipolar lacunar spinels, we find indications for dipolar relaxation dynamics at low temperatures. Polarization measurements on GaNb4Se8 reveal weak ferroelectric ordering below the magneto-structural transition, either superimposed to antipolar order or emerging at structural domain walls. The temperature-dependent dc resistivity evidences essentially thermally-activated charge transport with different activation energies in the different phases. A huge step-like increase of the resistivity at the magneto-structural transition of the Ta compound points to a fundamental change in the electronic structure or the mechanism of the charge transport. At low temperatures, charge transport is governed by in-gap impurity states, as also invoked to explain the resistive switching in these compounds.",2206.15200v2 2022-11-16,Decoupling the Roles of Defects/Impurities and Wrinkles in Thermal Conductivity of Wafer-scale hBN Films,"We demonstrate a non-monotonic evolution of thermal conductivity of large-area hexagonal boron nitride films with thickness. Wrinkles and defects/impurities are present in these films. Raman spectroscopy, an optothermal non-contact technique, is employed to probe the temperature and laser power dependence property of the Raman active E2ghigh phonon mode, which in turn is used to estimate the rise in the temperature of the films under different laser powers. As the conventional Fourier law of heat diffusion cannot be directly employed analytically to evaluate the thermal conductivity of these films with defects and wrinkles, finite element modeling is used instead. In the model, average heat resistance is used to incorporate an overall defect structure, and Voronoi cells with contact resistance at the cell boundaries are constructed to mimic the wrinkled domains. The effective thermal conductivity is estimated to be 87, 55, and 117 W/m.K for the 2, 10, and 30 nm-thick films, respectively. We also present a quantitative estimation of the thermal resistance by defects and wrinkles individually to the heat flow. Our study reveals that the defects/impurities render a much higher resistance to heat transfer in the films than wrinkles.",2211.08683v2 2022-11-18,Magnetotransport induced by anomalous Hall effect,"In a magnetic metal, the Hall resistance is generally taken to be the sum of the ordinary Hall resistance and the anomalous Hall resistance. Here it is shown that this empirical relation is no longer valid when either the ordinary Hall angle or the anomalous Hall angle is not small. Using the proper conductivity relation, we reveal an unexpected magnetoresistance (MR) induced by the anomalous Hall effect (AHE). A $B$-linear MR arises and the sign of the slope depends on the sign of the anomalous Hall angle, giving rise to a characteristic bowtie shape. The Hall resistance in a single-band system can exhibit a nonlinearity which is usually considered as a characteristic of a two-band system. A $B$-symmetric component appears in the Hall. These effects reflect the fundamental difference between the ordinary Hall effect and the AHE. Furthermore, we experimentally reproduce the unusual MR and Hall reported before in Co$_3$Sn$_2$S$_2$ and show that these observations can be well explained by the proposed mechanism. MR often observed in quantum anomalous Hall insulators provides further confirmation of the picture. The effect may also account for the large MR observed in non-magnetic three-dimensional topological Dirac semimetals.",2211.10222v2 2022-12-08,Theory of the Little-Parks effect in spin-triplet superconductors,"The celebrated Little-Parks effect in mesoscopic superconducting rings has recently gained great attention due to its potential to probe half-quantum vortices in spin-triplet superconductors. However, despite the large number of works reporting anomalous Little-Parks measurements attributed to unconventional superconductivity, the general signatures of spin-triplet pairing in the Little-Parks effect have not yet been systematically investigated. Here we use Ginzburg-Landau theory to study the Little-Parks effect in a spin-triplet superconducting ring that supports half-quantum vortices; we calculate the field-induced Little-Parks oscillations of both the critical temperature itself and the residual resistance resulting from thermal vortex tunneling below the critical temperature. We observe two separate critical temperatures with a single-spin superconducting state in between and find that, due to the existence of half-quantum vortices, each minimum in the upper critical temperature splits into two minima for the lower critical temperature. From a rigorous calculation of the residual resistance, we confirm that these two minima in the lower critical temperature translate into two maxima in the residual resistance below and establish the general conditions under which the two maxima can be practically resolved. In particular, we identify a fundamental trade-off between sharpening each maximum and keeping the overall magnitude of the resistance large. Our results will guide experimental efforts in designing mesoscopic ring geometries for probing half-quantum vortices in spin-triplet candidate materials on the device scale.",2212.04591v1 2023-04-16,Anomalous and Topological Hall Resistivity in Ta/CoFeB/MgO Magnetic Systems for Neuromorphic Computing Applications,"Topologically protected spin textures, such as magnetic skyrmions, have the potential for dense data storage as well as energy-efficient computing due to their small size and a low driving current. The evaluation of the writing and reading of the skyrmion's magnetic and electrical characteristics is a key step toward the implementation of these devices. In this paper, we present the magnetic heterostructure Hall bar device and study the anomalous Hall and topological Hall signals in the device. Using the combination of different measurements like magnetometry at different temperatures, Hall effect measurement from 2K to 300K, and magnetic force microscopy imaging, we investigate the magnetic and electrical characteristics of the magnetic structure. We measure the skyrmion topological resistivity at different temperatures as a function of the magnetic field. The topological resistivity is maximum around the zero magnetic field and it decreases to zero at the saturating field. This is further supported by MFM imaging. Interestingly the resistivity decreases linearly with the field, matching the behavior observed in the corresponding micromagnetic simulations. We combine the experimental results with micromagnetic simulations, thus propose a skyrmion-based synaptic device and show spin-orbit torque-controlled potentiation/depression in the device. The device performance as the synapse for neuromorphic computing is further evaluated in a convolutional neural network CNN. The neural network is trained and tested on the MNIST data set we show devices acting as synapses achieving a recognition accuracy close to 90%, on par with the ideal software-based weights which offer an accuracy of 92%.",2304.07742v1 2023-09-01,Multilayer Ferromagnetic Spintronic Devices for Neuromorphic Computing Applications,"Spintronics has gone through substantial progress due to its applications in energy-efficient memory, logic and unconventional computing paradigms. Multilayer ferromagnetic thin films are extensively studied for understanding the domain wall and skyrmion dynamics. However, most of these studies are confined to the materials and domain wall/skyrmion physics. In this paper, we present the experimental and micromagnetic realization of a multilayer ferromagnetic spintronic device for neuromorphic computing applications. The device exhibits multilevel resistance states and the number of resistance states increases with lowering temperature. This is supported by the multilevel magnetization behavior observed in the micromagnetic simulations. Furthermore, the evolution of resistance states with spin-orbit torque is also explored in experiments and simulations. Using the multi-level resistance states of the device, we propose its applications as a synaptic device in hardware neural networks and study the linearity performance of the synaptic devices. The neural network based on these devices is trained and tested on the MNIST dataset using a supervised learning algorithm. The devices at the chip level achieve 90\% accuracy. Thus, proving its applications in neuromorphic computing. Furthermore, we lastly discuss the possible application of the device in cryogenic memory electronics for quantum computers.",2309.00476v1 2024-01-30,Effect of the Sc/Zr ratio on the corrosion resistance of Al-Mg cast alloys,"The results of investigations of the corrosion resistance of Al-Mg-Sc-Zr alloys with varying Mg content and different Sc/Zr ratios are presented. The objects of investigations were the Al-Mg-Sc-Zr alloys with total Sc + Zr content of 0.32 wt%. The concentration of Sc and Zr in the alloys varied with the increments of 0.02 wt%. The alloys were produced by induction casting. The effect of annealing temperature on the microhardness and electrical resistivity of the Al-Mg-Sc-Zr alloys was investigated. Corrosion tests were carried out in a medium simulating intergranular corrosion in aluminum alloys. Electrochemical studies and mass loss tests were performed. An increase in the Sc concentration and a decrease in the Zr one were shown to result in an increase in the corrosion rate. The primary Al3(ScxZr1-x) particles were found to have the main effect on the corrosion resistance of Al-Mg-Sc-Zr alloys. The dependence of the corrosion current on the annealing temperature of the Al-Mg-Sc-Zr alloy was found to have a non-monotonous character (with a maximum).",2401.17429v1 1997-02-27,High temperature anomaly of the conductance of a tunnel junction,"The linear conductance of a tunnel junction in series with an ohmic resistor is determined in the high temperature limit. The tunneling current is treated nonperturbatively by means of path integral techniques. Due to quantum effects the conductance is smaller than the classical series conductance. The reduction factor is found to be nonanalytic in the environmental resistance for vanishing resistance. This behavior is a high temperature manifestation of the Coulomb blockade effect.",9702242v3 2002-10-11,High-field side of Superconductor-Insulator Transition,"We report the experimental observation of a magnetic-field-tuned superconductor-insulator transition (SIT) in ultrathin TiN films. The low temperature transport properties of these films show scaling behavior consistent with a transition driven by quantum phase fluctuations in two-dimensional superconductor. The magnetoresistance reveals peak and a subsequent decrease in fields higher than the critical field. The temperature dependences of the isomagnetic resistance data on the high-field side of the SIT have been analyzed and the transition from insulating to metallic phase is found, with at high fields the zero-temperature asymptotic value of the resistance being equal to h/e^2.",0210250v1 2003-11-11,Nonlocal effects in high energy charged particle beams,"Within the framework of the thermal wave model, an investigation is made of the longitudinal dynamics of high energy charged particle beams. The model includes the self-consistent interaction between the beam and its surroundings in terms of a nonlinear coupling impedance, and when resistive as well as reactive parts are included, the evolution equation becomes a generalised nonlinear Schroedinger equation including a nonlocal nonlinear term. The consequences of the resistive part on the propagation of particle bunches are examined using analytical as well as numerical methods.",0311139v1 2008-11-05,"High-pressure, transport, and thermodynamic properties of CeTe3","We have performed high-pressure, electrical resistivity, and specific heat measurements on CeTe3 single crystals. Two magnetic phases with nonparallel magnetic easy axes were detected in electrical resistivity and specific heat at low temperatures. We also observed the emergence of an additional phase at high pressures and low temperatures and a possible structural phase transition detected at room temperature and at 45 kbar, which can possibly be related with the lowering of the charge-density wave transition temperature known for this compound.",0811.0792v2 2009-07-30,High order fractional microwave induced resistance oscillations in 2D systems,"We report on the observation of microwave-induced resistance oscillations associated with the fractional ratio n/m of the microwave irradiation frequency to the cyclotron frequency for m up to 8 in a two-dimensional electron system with high electron density. The features are quenched at high microwave frequencies independent of the fractional order m. We analyze temperature, power, and frequency dependencies of the magnetoresistance oscillations and discuss them in connection with existing theories.",0907.5315v1 2010-11-24,A spark-resistant bulk-micromegas chamber for high-rate applications,"We report on the design and performance of a spark-resistant bulk-micromegas chamber. The principle of this design lends itself to the construction of large-area muon chambers for the upgrade of the detectors at the Large Hadron Collider at CERN for luminosities in excess of 10**34/cm2/s or other high-rate applications.",1011.5370v1 2012-12-10,Quantized escape and formation of edge channels at high Landau levels,"We present nonlocal resistance measurements in an ultra high mobility two dimensional electron gas. Our experiments show that even at weak magnetic fields classical guiding along edges leads to a strong non local resistance on macroscopic distances. In this high Landau level regime the transport along edges is dissipative and can be controlled by the amplitude of the voltage drop along the edge. We report resonances in the nonlocal transport as a function of this voltage that are interpreted as escape and formation of edge channels.",1212.2026v1 2019-06-26,Studies on small charge packet transport in high-resistivity fully-depleted CCDs,"In this work, we will present a physical model and measurements of the transport of small charge packets in the bulk of thick high resistivity CCD before being collected by the pixel potential wells. A new technique to measure the lateral spread of the charge as a function of the ionization depth in the bulk is presented. Results from measurements on CCD currently in use for several scientific instruments are shown and validated with a new mathematical algorithm to extend the current modeling based only on the diffusion of the charge in silicon.",1906.11379v1 2011-07-09,Resistance to TB drugs in KwaZulu-Natal: causes and prospects for control,"In 2005 there was an outbreak of XDR (extensively drug resistant) TB in Tugela Ferry, which is served by the Church of Scotland Hospital (COSH), in the uMzinyathi District, KwaZulu-Natal, South Africa. An investigation was carried out to determine if XDR TB was occurring elsewhere in the province, and to develop hypotheses for the rise in drug resistance with a view to developing a strategy for the control of MDR (multi-drug resistant) and XDR TB in the province and elsewhere. TB incidence and treatment success rates, for each of the 11 districts in the province, were obtained from the provincial electronic TB register for the years 2002-2007. The results of culture and drug sensitivity tests for the years 2002 to 2007 in each of the districts were compiled and culture taking practices were compared to the number of MDR TB cases. Interviews were conducted with key personnel in affected sites. In 2007, 2799, or 2.3% of 119,218 notified TB cases in the province were multi-drug resistant (MDR), and of these 270 (9.6%) were XDR. The two worst affected districts were uMzinyathi where 226 (4.1%) of 5522 notified TB cases were MDR, and of these 120 (53%) were extensively drug resistant (XDR), and uMkhanyakude where 337 (4.8%) of 6991 notified TB cases were MDR, but of these only four or (1.2%) were XDR. The worst affected medical centre was COSH where 164 or 9.8% of notified TB cases were MDR and of these 99 (60%) were XDR. Very high rates of XDR TB in the province are only found in uMzinyathi district even though MDR TB is common in most other districts. XDR may arisen at COSH because of the early and effective integration of the TB and HIV programmes in overcrowded and poorly ventilated facilities particular to COS.H To control XDR TB better management of both susceptible and resistant forms of TB is needed including treatment supervision, infection control and HIV management.",1107.1800v1 2012-02-06,Performances of Anode-resistive Micromegas for HL-LHC,"Micromegas technology is a promising candidate to replace Atlas forward muon chambers -tracking and trigger- for future HL-LHC upgrade of the experiment. The increase on background and pile-up event probability requires detector performances which are currently under studies in intensive RD activities. We studied performances of four different resistive Micromegas detectors with different read-out strip pitches. These chambers were tested using \sim120 GeV momentum pions, at H6 CERN-SPS beam line in autumn 2010. For a strip pitch 500 micrometers we measure a resolution of \sim90 micrometers and a efficiency of ~98%. The track angle effect on the efficiency was also studied. Our results show that resistive techniques induce no degradation on the efficiency or resolution, with respect to the standard Micromegas. In some configuration the resistive coating is able to reduce the discharge currents at least by a factor of 100.Micromegas technology is a promising candidate to replace Atlas forward muon chambers -tracking and trigger- for future HL-LHC upgrade of the experiment. The increase on background and pile-up event probability requires detector performances which are currently under studies in intensive RD activities. We studied performances of four different resistive Micromegas detectors with different read-out strip pitches. These chambers were tested using \sim120 GeV momentum pions, at H6 CERN-SPS beam line in autumn 2010. For a strip pitch 500 micrometers we measure a resolution of \sim90 micrometers and a efficiency of \sim98%. The track angle effect on the efficiency was also studied. Our results show that resistive techniques induce no degradation on the efficiency or resolution, with respect to the standard Micromegas. In some configuration the resistive coating is able to reduce the discharge currents at least by a factor of 100.",1202.1074v1 2018-11-12,Phonon-induced giant linear-in-$T$ resistivity in magic angle twisted bilayer graphene: Ordinary strangeness and exotic superconductivity,"We study the effect of electron-acoustic phonon interactions in twisted bilayer graphene on resistivity in the high-temperature transport and superconductivity in the low-temperature phase diagram. We theoretically show that twisted bilayer graphene should have an enhanced and strongly twist-angle dependent linear-in-temperature resistivity in the metallic regime with the resistivity magnitude increasing as the twist angle approaches the magic angle. The slope of the resistivity versus temperature could approach one hundred ohms per kelvin with a strong angle dependence, but with a rather weak dependence on the carrier density. This higher-temperature density-independent linear-in-$T$ resistivity crosses over to a $T^4$ dependence at a low density-dependent characteristic temperature, becoming unimportant at low temperatures. This angle-tuned resistivity enhancement arises from the huge increase in the effective electron-acoustic phonon coupling in the system due to the suppression of graphene Fermi velocity induced by the flatband condition in the moir\'e superlattice system. Our calculated temperature dependence is reminiscent of the so-called `strange metal' transport behavior except that it is arising from the ordinary electron-phonon coupling in a rather unusual parameter space due to the generic moir\'e flatband structure of twisted bilayer graphene. We also show that the same enhanced electron-acoustic phonon coupling also mediates effective attractive interactions in $s$, $p$, $d$ and $f$ pairing channels with a theoretical superconducting transition temperature on the order of $\sim$5 K near magic angle. The fact that ordinary acoustic phonons can produce exotic non-$s$-wave superconducting pairing arises from the unusual symmetries of the system.",1811.04920v4 2017-03-07,A Strange Metal from Gutzwiller correlations in infinite dimensions,"Recent progress in extremely correlated Fermi liquid theory (ECFL) and dynamical mean field theory (DMFT) enables us to compute in the $d \to \infty$ limit the resistivity of the $t-J$ model after setting $J\to0$. This is also the $U=\infty$ Hubbard model. We study three densities $n=.75,.8,.85$ that correspond to a range between the overdoped and optimally doped Mott insulating state. We delineate four distinct regimes characterized by different behaviors of the resistivity $\rho$. We find at the lowest $T$ a Gutzwiller Correlated Fermi Liquid regime with $\rho \propto T^2$ extending up to an effective Fermi temperature that is dramatically suppressed from the non-interacting value. This is followed by a Gutzwiller Correlated Strange Metal regime with $\rho \propto (T-T_0)$, i.e. a linear resistivity extrapolating back to $\rho=0$ at a positive $T_0$. At a higher $T$ scale, this crosses over into the Bad Metal regime with $\rho \propto (T+T_1)$ extrapolating back to a finite resistivity at $T=0$, and passing through the Ioffe-Regel-Mott value where the mean free path is a few lattice constants. This regime finally gives way to the High $T$ Metal regime, where we find $\rho \propto T$. The present work emphasizes the first two, where the availability of an analytical ECFL theory is of help in identifying the changes in related variables entering the resistivity formula that accompany the onset of linear resistivity, and the numerically exact DMFT helps to validate the results. We also examine thermodynamic variables such as the magnetic susceptibility, compressibility, heat capacity and entropy, and correlate changes in these with the change in resistivity. This exercise casts valuable light on the nature of charge and spin correlations in the strange metal regime, which has features in common with the physically relevant strange metal phase seen in strongly correlated matters.",1703.02206v3 2019-07-16,General relativistic resistive magnetohydrodynamics with robust primitive variable recovery for accretion disk simulations,"Recent advances in black hole astrophysics, particularly the first visual evidence of a supermassive black hole at the center of the galaxy M87 by the Event Horizon Telescope (EHT), and the detection of an orbiting ""hot spot"" nearby the event horizon of Sgr A* in the Galactic center by the Gravity Collaboration, require the development of novel numerical methods to understand the underlying plasma microphysics. Non-thermal emission related to such hot spots is conjectured to originate from plasmoids that form due to magnetic reconnection in thin current layers in the innermost accretion zone. Resistivity plays a crucial role in current sheet formation, magnetic reconnection, and plasmoid growth in black hole accretion disks and jets. We included resistivity in the three-dimensional general-relativistic magnetohydrodynamics (GRMHD) code BHAC and present the implementation of an Implicit-Explicit scheme to treat the stiff resistive source terms of the GRMHD equations. The algorithm is tested in combination with adaptive mesh refinement to resolve the resistive scales and a constrained transport method to keep the magnetic field solenoidal. Several novel methods for primitive variable recovery, a key part in relativistic magnetohydrodynamics codes, are presented and compared for accuracy, robustness, and efficiency. We propose a new inversion strategy that allows for resistive-GRMHD simulations of low gas-to-magnetic pressure ratio and highly magnetized regimes as applicable for black hole accretion disks, jets, and neutron star magnetospheres. We apply the new scheme to study the effect of resistivity on accreting black holes, accounting for dissipative effects as reconnection.",1907.07197v2 2020-06-23,Thermal interfacial resistance and nanolayer effect on the thermal conductivity of Al2O3-CO2 nanofluid: A Molecular Dynamics approach,"Nanofluids are known to have significantly different thermal properties relative to the corresponding conventional fluids. Heat transfer at the solid-fluid interface affects the thermal properties of nanofluids. The current work helps in understanding the role of two nanoscale phenomena, namely ordering of fluid layer around the nanoparticle (nanolayer) and thermal resistance at the interface of solid-fluid in the enhancement of thermal conductivity of Al2O3 - CO2 nanofluid. In this study, molecular dynamics (MD) simulations have been used to study the thermal interfacial resistance by transient non-equilibrium heat technique and nanolayer formed between Al2O3 nanoparticle (np) and surrounded CO2 molecules in the gaseous and supercritical phase. The nanoparticle diameter (dNP) is varied between 2 and 5 nm to investigate the size effect on thermal interfacial resistance (TIR) and thermal conductivity of nanofluid and the results indicate that the TIR for larger diameters is relatively high in both the phases. The study of the effect of surface wettability and temperature on TIR reveals that the resistance decreases with increase in interaction strength and temperature, but is entirely independent at higher temperatures, in both gaseous and supercritical nanofluid. A density distribution study of the nanolayer and the monolayer around the nanoparticle revealed that the latter is more ordered in smaller diameter with less thermal resistance. However, nanolayer study reveals that the nanoparticle with bigger diameters are more suitable for the cooling/heating purpose, as the system with larger diameters has higher thermal conductivity. Results show that the nanolayer plays a significant role in determining the effective thermal conductivity of the nanofluid, while the influence of TIR appears negligible compared to the nanolayer.",2006.12805v2 2022-03-12,Parameterization of hydrodynamic friction in a model for sheared suspensions of rough particles,"We propose a method to parameterize a coarse grained model for the hydrodynamic friction between nearly touching rough spheres in suspension flows. The frictional resistance due to surface roughness primarily alters the sliding and rolling modes of motion of rough particles. Stokesian dynamics simulations incorporating a near-field pairwise resistance model accounting for these enhanced frictional modes were employed to compute particle trajectories in shear flow. In this model, the resistance to sliding and rolling modes of motion are augmented from a weakly diverging log$(1/h)$ form for smooth spheres to a strongly diverging $1/h$ form for rough spheres to account for the additional resistance due to squeezing flows between surface asperities, where $h$ is the mean surface separation between particles. We determine new bounds on the relative magnitude of the augmentations to the resistance to different modes of motion using inequality constraints reflecting the positive definiteness of the Stokes resistance tensor for a pair of rough particles. Using the simulations of a particle pair in a shear flow, a simple model for angular rotation rate of the pair centerline is computed as a function of its orientation in the shear flow and the free parameters of the hydrodynamic resistance model: the friction coupling strength, $\alpha$, and friction coupling range, $h_0$. Values of $\alpha$ and $h_0$ for real-world rough particles can then be inferred by matching the pair rotation rate in the model to experimental observations when a dilute rough particle suspension is subjected to a linear shear flow. The same model is used to calculate the hydrodynamic contribution to the high frequency viscosity of rough particle suspensions. For different $\alpha$ and $h_0$, we observe that the viscosity diverges differently depending on $h_0$.",2203.06300v1 2003-11-17,Collapse of Magnetized Singular Isothermal Toroids: I. Non-Rotating Case,"We study numerically the collapse of non-rotating, self-gravitating, magnetized, singular isothermal toroids characterized by sound speed, $a$, and level of magnetic to thermal support, $H_0$. In qualitative agreement with previous treatments by Galli & Shu and other workers, we find that the infalling material is deflected by the field lines towards the equatorial plane, creating a high-density, flattened structure -- a pseudodisk. The pseudodisk contracts dynamically in the radial direction, dragging the field lines threading it into a highly pinched configuration that resembles a split monopole. The oppositely directed field lines across the midplane and the large implied stresses may play a role in how magnetic flux is lost in the actual situation in the presence of finite resistivity or ambipolar diffusion. The infall rate into the central regions is given to 5% uncertainty by the formula, $\dot M = (1+H_0)a^3/G$, where $G$ is the universal gravitational constant, anticipated by semi-analytical studies of the self-similar gravitational collapses of the singular isothermal sphere and isopedically magnetized disks. The introduction of finite initial rotation results in a complex interplay between pseudodisk and true (Keplerian) disk formation that is examined in a companion paper.",0311376v1 2006-02-01,From Protoplanets to Protolife: The Emergence and Maintenance of Life,"Despite great advances in our understanding of the formation of the Solar System, the evolution of the Earth, and the chemical basis for life, we are not much closer than the ancient Greeks to an answer of whether life has arisen and persisted on any other planet. The origin of life as a planetary phenomenon will probably resist successful explanation as long as we lack an early record of its evolution and additional examples. It is widely thought that the geologic record shows that life emerged quickly after the end of prolonged bombardment of the Earth. New data and simulations contradict that view and suggest that more than half a billion years of unrecorded Earth history may have elapsed between the origin of life and LUCA. The impact-driven exchange of material between the inner planets may have allowed earliest life to be more cosmopolitan. Indeed, terrestrial life may not have originated on the Earth, or even on any planet. Smaller bodies, e.g. the parent bodies of primitive meteorites, offer alternative environments for the origin of life in our Solar System. The search for past or present life on Mars is an obvious path to greater enlightenment. The subsurface oceans of some icy satellites of the outer planets represent the best locales to search for an independent origin of life in the Solar System because of the high dynamical barriers for transfer, intense radiation at their surfaces, and thick ice crusts. The ``ultimate'' answer to the abundance of life in the Cosmos will remain the domain of speculation until we develop observatories capable of detecting habitable planets - and signs of life - around the nearest million or so stars.",0602008v1 2000-05-10,"Magnetic, thermal, and transport properties on single crystals of antiferromagnetic Kondo-lattice Ce2PdSi3","Magnetization, heat capacity, electrical resistivity, thermoelectric power, and Hall effect have been investigated on single-crystalline Ce_2PdSi_3. This compound is shown to order antiferromagnetically below N'eel temperature (T_N) \~3 K. The Sommerfeld coefficient far below T_N is found to be about 110 mJ/K^2 mol Ce, which indicates the heavy-fermion character of this compound. The transport and magnetic properties exhibit large anisotropy with an interplay between crystalline-electric-field (CEF) and Kondo effects. The sign of thermoelectric power is opposite for different directions at high temperatures and the ordinary Hall coefficient is anisotropic with opposite sign for different geometries, indicating the anisotropic Fermi surface. The CEF analysis from the temperature dependence of magnetic susceptibility suggests that the ground state is |+/-1/2>. The first and the second excited CEF doublet levels are found to be located at about 30 and 130 K, respectively. The Kondo temperature is estimated to be the same order as T_N, indicating the presence of a delicate competition between the Kondo effect and magnetic order.",0005164v1 2001-06-03,Transport processes in metal-insulator granular layers,"The non-equilibrium tunnel transport processes are considered in a square lattice of metallic nanogranules embedded into insulating host. Based on a simple model with three possible charging states (+,-, or 0) of a granule and three kinetic processes (creation or recombination of a +- pair, and charge transfer) between neighbor granules, the mean-field kinetic theory is developed, which takes into account the interplay between the charging energy and temperature and between the applied electric field and Coulomb fields by non-compensated charge density. The resulting charge and current distributions are found to depend essentially on the particular conditions in a granular layer, namely, in a free area (FA) or in contact areas (CA) under macroscopic metallic contacts. Thus, a steady state dc transport is only compatible with zero charge density and ohmic resistivity within FA, but charge accumulation and non-ohmic behavior are necessary for conduction over CA. The approximate analytic solutions are obtained for characteristic regimes (low or high charge density) of such conduction. Also non- stationary processes are considered, displaying a peculiar combination of two strongly different relaxation times. The comparison is done with the available transport data on similar experimental systems.",0106034v2 2002-03-06,Concentration Dependence of Superconductivity and Order-Disorder Transition in the Hexagonal Rubidium Tungsten Bronze RbxWO3. Interfacial and bulk properties,"We revisited the problem of the stability of the superconducting state in RbxWO3 and identified the main causes of the contradictory data previously published. We have shown that the ordering of the Rb vacancies in the nonstoichiometric compounds have a major detrimental effect on the superconducting temperature Tc.The order-disorder transition is first order only near x = 0.25, where it cannot be quenched effectively and Tc is reduced below 1K. We found that the high Tc's which were sometimes deduced from resistivity measurements, and attributed to compounds with .25 < x < .30, are to be ascribed to interfacial superconductivity which generates spectacular non-linear effects. We also clarified the effect of acid etching and set more precisely the low-rubidium-content boundary of the hexagonal phase.This work makes clear that Tc would increase continuously (from 2 K to 5.5 K) as we approach this boundary (x = 0.20), if no ordering would take place - as its is approximately the case in CsxWO3. This behaviour is reminiscent of the tetragonal tungsten bronze NaxWO3 and asks the same question : what mechanism is responsible for this large increase of Tc despite the considerable associated reduction of the electron density of state ? By reviewing the other available data on these bronzes we conclude that the theoretical models which are able to answer this question are probably those where the instability of the lattice plays a major role and, particularly, the model which call upon local structural excitations (LSE), associated with the missing alkali atoms.",0203120v1 2003-04-19,Transport properties of granular metals at low temperatures,"We investigate transport in a granular metallic system at large tunneling conductance between the grains, $g_T\gg 1$. We show that at low temperatures, $T\leq g_T\delta $, where $\delta$ is the single mean energy level spacing in a grain, the coherent electron motion at large distances dominates the physics, contrary to the high temperature ($T>g_T\delta $) behavior where conductivity is controlled by the scales of the order of the grain size. The conductivity of one and two dimensional granular metals, in the low temperature regime, decays with decreasing temperature in the same manner as that in homogeneous disordered metals, indicating thus an insulating behavior. However, even in this temperature regime the granular structure remains important and there is an additional contribution to conductivity coming from short distances. Due to this contribution the metal-insulator transition in three dimensions occurs at the value of tunnel conductance $g_T^C=(1/6\pi)\ln (E_C/\delta)$, where $E_C$ is the charging energy of an isolated grain, and not at the generally expected $g_T^C\propto 1$. Corrections to the density of states of granular metals due to the electron-electron interaction are calculated. Our results compare favorably with the logarithmic dependence of resistivity in the high-$T_c$ cuprate superconductors indicating that these materials may have a granular structure.",0304448v1 2004-03-31,Correlation of microwave surface impedance of MgB_2 thin film with material parameters and a temperature niche for microwave applications,"Two issues related to the microwave surface impedance Z_s of MgB_2 thin film are discussed in this Letter, both being significant for potential microwave applications. At first, a correlation between Zs and Alpha = Xi/l was found, where Xi is the coherence length, and l is the mean free path. The surface resistance Rs decreases with Alpha at moderate and large values of Alpha and saturates when Alpha approaches one. The values of the penetration depth at zero temperature Lamda(0) for different films could be well fitted by Lamda_L (1+Alpha)^(1/2), yielding a London penetration depth Lamda_L of 33.6 nm. The second issue is to find a temperature niche for possible microwave applications. Between 10K and 15K, our best MgB_2 films possess the lowest Rs values compared with other superconductors such as NbN, Nb3Sn and the high-temperature superconductor YBCO.",0403755v1 2004-10-21,Effect of nanometer-sized B powder on phase formation of polycrystalline MgB2,"The size effect of the raw B powder on the MgB2 phase formation has been studied by the technique of in-situ high temperature resistivity (HT-rT) measurement. The onset temperature, Tonset, and the completion temperature, TPF, of the phase formation are determined directly during the ongoing thermal process. These two temperatures, Tonset and TPF of the sample synthesized using nanometer B and Mg powders (NanoB-MgB2) are 440 C and 490 C, respectively, the same as those of the sample using micrometer B and nanometer Mg powders (MicroB-MgB2). This indicates that the phase formation temperature of MgB2 do not depend on the B powder size. On the other hand, the upper limit of the sintering temperature, TN, above which the sample loses superconductivity, is below 750 C for NanoB-MgB2, much lower than 980 C for the MgB2 prepared using micron-sized B powder and millimeter sized Mg powder (DM-MgB2). In comparison with the sample directly sintered at 650 C < TN, an interesting, irreversible transformation in the crystal structure of the MgB2 phase was observed with the sample going through the stages of initial sintering at 750 C, then re-sintering at 650 C in an Mg-rich environment after the processes of regrinding and pressing. Possible explanation of the observed properties is discussed.",0410533v1 2005-03-18,Aharonov-Bohm electron interferometer in the integer quantum Hall regime,"We report experiments on a quantum electron interferometer fabricated from high mobility, low density GaAs/AlGaAs heterostructure material. In this device, a nearly circular electron island is defined by four front gates deposited in etched trenches. The island is separated from the 2D electron bulk by two nearly open constrictions. In the quantum Hall regime, two counterpropagating edge channels are coupled by tunneling in the constrictions, thus forming a closed electron interference path.For several fixed front gate voltages, we observe periodic Aharonov-Bohm interference oscillations in four-terminal resistance as a function of the enclosed flux. The oscillation period DeltaB gives the area of the interference path S via quantization condition S=h/eDeltaB. We experimentally determine the dependence of S on the front gate voltage, and find that the Aharonov-Bohm quantization condition does not require significant corrections due to the confining potential. These results can be interpreted as a constant integrated compressibility of the island with respect to the front gates. We also analyze experimental results using two classical electrostatics models: one modeling the 2D electron density due to depletion from an etch trench, and another modeling the gate voltage dependence of the electron density profile in the island.",0503456v2 2006-09-05,Electrical and Thermal Transport in Metallic Single-Wall Carbon Nanotubes on Insulating Substrates,"We analyze transport in metallic single-wall carbon nanotubes (SWNTs) on insulating substrates over the bias range up to electrical breakdown in air. To account for Joule self-heating, a temperature-dependent Landauer model for electrical transport is coupled with the heat conduction equation along the nanotube. The electrical breakdown voltage of SWNTs in air is found to scale linearly with their length, approximately as 5 V/um; we use this to deduce a thermal conductance between SWNT and substrate g ~ 0.17 +/- 0.03 W/K/m per tube length, which appears limited by the SWNT-substrate interface rather than the thermal properties of the substrate itself. We examine the phonon scattering mechanisms limiting electron transport, and find the strong temperature dependence of the optical phonon absorption rate to have a remarkable influence on the electrical resistance of micron-length nanotubes. Further analysis reveals that unlike in typical metals, electrons are responsible for less than 15% of the total thermal conductivity of metallic nanotubes around room temperature, and this contribution decreases at high bias or higher temperatures. For interconnect applications of metallic SWNTs, significant self-heating may be avoided if power densities are limited below 5 uW/um, or if the SWNT-surrounding thermal interface is optimized.",0609075v2 2009-09-14,Progress in the development of a S RETGEM-based detector for an early forest fire warning system,"In this paper we present a prototype of a Strip Resistive Thick GEM photosensitive gaseous detector filled with Ne and ethylferrocene vapours at a total pressure of 1 atm for an early forest fire detection system. Tests show that it is one hundred times more sensitive than the best commercial ultraviolet flame detectors and therefore, it is able to reliably detect a flame of 1.5x1.5x1.5 m3 at a distance of about 1km. An additional and unique feature of this detector is its imaging capability, which in combination with other techniques, may significantly reduce false fire alarms when operating in an automatic mode. Preliminary results conducted with air filled photosensitive gaseous detectors are also presented. The approach main advantages include both the simplicity of manufacturing and affordability of construction materials such as plastics and glues specifically reducing detector production cost. The sensitivity of these air filled detectors at certain conditions may be as high as those filled with Ne and EF. Long term test results of such sealed detectors indicate a significant progress in this direction. We believe that our detectors utilized in addition to other flame and smoke sensors will exceptionally increase the sensitivity of forest fire detection systems. Our future efforts will be focused on attempts to commercialize such detectors utilizing our aforementioned findings.",0909.2480v1 2009-09-28,Hall effect in superconducting Fe(Se0.5Te0.5) thin films,"The Hall effect is investigated for eight superconducting Fe(Se_0.5_Te_0.5_) thin films grown on MgO and LaSrAlO_4_ substrates with different transition temperatures (T_c_). The normal Hall coefficients (R_H_) have positive values with magnitude of 1 - 1.5 x 10^-3^ cm^3^/C at room temperature for the all samples. With decreasing temperature, we find two characteristic types of behavior in R_H_(T) depending on T_c_. For thin films with lower T_c_ (typically T_c_ < 5 K), R_H_ start decreasing approximately below T = 250 K toward a negative side, some of which shows sign reversal at T = 50 - 60 K, but turns positive toward T = 0 K. On the other hand for the films with higher T_c_ (typically T_c_ > 9 K), R_ H_ leaves almost unchanged down to T = 100 K, and then starts decreasing toward a negative side. Around the temperatures when R_H_ changes its sign from positive to negative, obvious nonlinearity is observed in the field-dependence of Hall resistance as to keep the low-field R_H_ positive while the high-field R_H_ negative. Thus the electronic state just above T_c_ is characterized by n_e_ (electron density) > n_h_ (hole density) with keeping \mu_e_ < \mu_h_. These results suggest the dominance of electron density to the hole density is an essential factor for the occurence of superconductivity in Fe-chalcogenide superconductors.",0909.4985v3 2010-11-14,Tunneling anisotropic magnetoresistance of NiFe/IrMn/MgO/Pt stack: An antiferromagnet based spin-valve,"Spin-valve is a microelectronic device in which high and low resistance states are realized by utilizing both charge and spin of carriers. Spin-valve structures used in modern hard drive read-heads and magnetic random access memories comprise two ferromagnetic (FM) electrodes whose relative magnetization orientations can be switched between parallel and antiparallel configurations, yielding the desired giant or tunneling magnetoresistance effect. In this paper we demonstrate >100$% spin-valve-like signal in a NiFe/IrMn/MgO/Pt stack with an antiferromagnet (AFM) on one side and a non-magnetic metal on the other side of the tunnel barrier. FM moments in NiFe are reversed by external fields <50mT and the exchange-spring effect of NiFe on IrMn induces rotation of AFM moments in IrMn which is detected by the measured tunneling anisotropic magnetoresistance (TAMR). Our work demonstrates a spintronic element whose transport characteristics are governed by an AFM. It demonstrates that sensitivity to low magnetic fields can be combined with large, spin-orbit coupling induced magneto-transport anisotropy using a single magnetic electrode. The AFM-TAMR provides means to study magnetic characteristics of AFM films by an electronic transport measurement.",1011.3188v1 2011-09-09,Study of ageing in Al-Mg-Si alloys by positron annihilation spectroscopy,"In many common Al-Mg-Si alloys (6000 series) intermediate storage at or near 'room temperature' after solutionising leads to pronounced changes of the precipitation kinetics during the ensuing artificial ageing step at \approx 180{\deg}C. This is not only an annoyance in production, but also a challenge for researchers. We studied the kinetics of natural 'room temperature' ageing (NA) in Al-Mg-Si alloys by means of various different techniques, namely electrical resistivity and hardness measurement, thermoanalysis and positron lifetime and Doppler broadening (DB) spectroscopy to identify the stages in which the negative effect of NA on artificial ageing might appear. Positron lifetime measurements were carried out in a fast mode, allowing us to measure average lifetimes in below 1 minute. DB measurements were carried out with a single detector and a 68Ge positron source by employing high momentum analysis. The various measurements show that NA is much more complex than anticipated and at least four different stages can be distinguished. The nature of these stages cannot be given with certainty, but a possible sequence includes vacancy diffusion to individual solute atoms, nucleation of solute clusters, Mg agglomeration to clusters and coarsening or ordering of such clusters. Positron lifetime measurements after more complex ageing treatments involving storage at 0{\deg}C, 20{\deg}C and 180{\deg}C have also been carried out and help to understand the mechanisms involved.",1109.2019v2 2012-11-20,Enhanced superconducting performance of melt quenched Bi2Sr2CaCu2O8 (Bi-2212) superconductor,"We scrutinize the enhanced superconducting performance of melt quench Bismuth based Bi2Sr2CaCu2O8 (Bi-2212) superconductor. The superconducting properties of melt quenched Bi-2212 (Bi2212-MQ) sample are compared with non-melted Bi2212-NM and Bi1.4Pb0.6Sr2Ca2Cu3O10 (Bi-2223). Crystal structure and morphology of the samples are studied using X-ray diffraction and Scanning Electron Microscopy (SEM) techniques. The high field (14T) magneto-transport and DC/AC magnetic susceptibility techniques are extensively used to study the superconducting properties of the investigated samples. The superconducting critical temperature (Tc) and upper critical field (Hc2) as well as thermally activated flux flow (TAFF) activation energy are estimated from the magneto-resistive [R(T)H] measurements. Both DC magnetization and amplitude dependent AC susceptibility measurements are used to determine the field and temperature dependence of critical current density (Jc) for studied samples. On the other hand, the frequency dependent AC susceptibility is used for estimating flux creep activation energy. It is found that melt quenching significantly enhances the superconducting properties of granular Bi-2212 superconductor. The results are interpreted in terms of better alignment and inter-connectivity of the grains along with reduction of grain boundaries for Bi2212-MQ sample.",1211.4681v2 2013-07-27,Strain-induced effects on the magnetic and electronic properties of epitaxial Fe$_{1-x}$Co$_{x}$Si thin films,"We have investigated the Co-doping dependence of the structural, transport, and magnetic properties of \epsilon-FeCoSi epilayers grown by molecular beam epitaxy on silicon (111) substrates. Low energy electron diffraction, atomic force microscopy, X-ray diffraction, and high resolution transmission electron microscopy studies have confirmed the growth of phase-pure, defect-free \epsilon-FeCoSi epitaxial films with a surface roughness of ~1 nm. These epilayers are strained due to lattice mismatch with the substrate, deforming the cubic B20 lattice so that it becomes rhombohedral. The temperature dependence of the resistivity changes as the Co concentration is increased, being semiconducting-like for low $x$ and metallic-like for x \gtrsim 0.3. The films exhibit the positive linear magnetoresistance that is characteristic of \epsilon-FeCoSi below their magnetic ordering temperatures $T_\mathrm{ord}$, as well as the huge anomalous Hall effect of order several \mu\Omega cm. The ordering temperatures are higher than those observed in bulk, up to 77 K for x = 0.4. The saturation magnetic moment of the films varies as a function of Co doping, with a contribution of ~1 \mu_{B}/ Co atom for x \lesssim 0.25. When taken in combination with the carrier density derived from the ordinary Hall effect, this signifies a highly spin-polarised electron gas in the low x, semiconducting regime.",1307.7301v1 2013-08-05,"Enhancement of superconductivity near the pressure-induced semiconductor-metal transition in BiS2-based compounds LnO(0.5)F(0.5)BiS2 (Ln = La, Ce, Pr, Nd)","Measurements of electrical resistivity were performed between 3 and 300 K at various pressures up to 2.8 GPa on the BiS2-based superconductors LnO0.5F0.5BiS2 (Ln = Pr, Nd). At lower pressures, PrO0.5F0.5BiS2 and NdO0.5F0.5BiS2 exhibit superconductivity with critical temperatures Tc of 3.5 and3.9 K, respectively. As pressure is increased, both compounds undergo a transition at a pressure Pt from a low Tc superconducting phase to a high Tc superconducting phase in which Tc reaches maximum values of 7.6 and 6.4 K for PrO0.5F0.5BiS2 and NdO0.5F0.5BiS2, respectively. The pressure-induced transition is characterized by a rapid increase in Tc within a small range in pressure of ~0.3 GPa for both compounds. In the normal state of PrO0.5F0.5BiS2, the transition pressure Pt correlates with the pressure where the suppression of semiconducting behaviour saturates. In the normal state of NdO0.5F0.5BiS2, Pt is coincident with a semiconductor-metal transition. This behaviour is similar to the results recently reported for the LnO0.5F0.5BiS2 (Ln = La, Ce) compounds. We observe that Pt and the size of the jump in Tc between the two superconducting phases both scale with the lanthanide element in LnO0.5F0.5BiS2 (Ln = La, Ce, Pr, Nd).",1308.1072v3 2014-02-13,"Colloidal pattern replication through contact photolithography operated in a ""Talbot-Fabry-Perot"" regime","We detail on a continuous colloidal pattern replication by using contact photolithography. Chrome on quartz masks are fabricated using colloidal nanosphere lithography and subsequently used as photolithography stamps. Hexagonal pattern arrangements with different dimensions (980, 620 and 480 nm, using colloidal particles with respective diameters) have been studied. When the mask and the imaged resist layer were in intimate contact, a high fidelity pattern replica was obtained after photolithography exposure and processing. In turn, the presence of an air-gap in between has been found to affect the projected image onto the photoresist layer, strongly dependent on the mask feature size and air-gap height. Pattern replication, inversion and hybridization was achieved for 980 nm-period mask; no hybridization for the 620 nm; and only pattern replication for the 480 nm. These results are interpreted in the framework of a ""Talbot-Fabry-Perot"" effect. Numerical simulations corroborate with the experimental findings providing insight into the involved processes highlighting the important parameters affecting the exposure pattern. The approach allows complex subwavelength patterning and is relevant for a 3D layer-by-layer printing.",1402.3117v1 2014-02-28,Exploring of point-contact spectra of Ba1-xNaxFe2As2 in the normal and superconducting state,"We present study of derivatives of current-voltage I(V) characteristics of point-contacts (PCs) based on Ba{1-x}Na{x}Fe2As2 (x=0.25) in the normal and superconducting state. The detailed analysis of dV/dI(V) data (also given in Appendix A) shows that the thermal regime, when temperature increases with a voltage at a rate of about 1.8 K/mV, is realized in the investigated PCs at least at high biases V above the superconducting (SC) gap \Delta. In this case, specific resistivity \rho (T) in PC core is responsible for a peculiar dV/dI(V) behavior, while a pronounced asymmetry of dV/dI(V) is caused by large value of thermopower in this material. A reproducible zero-bias minima detected on dV/dI(V) at low biases in the range \pm(6--9)mV well below the SC critical temperature T_c could be connected with the manifestation of the SC gap \Delta. Evaluation of these Andreev-reflection-like structures on dV/dI(V) points out to the preferred value of 2\Delta/kT_c \approx 6. The expected second gap features on dV/dI(V) are hard to resolve unambiguously, likely due to impurity scattering, spatial inhomogeneity and transition to the mentioned thermal regime as the bias further increases. Suggestions are made how to separate spectroscopic features in dV/dI(V) from those caused by the thermal regime.",1402.7233v1 2014-03-16,Electrical Contacts to Three-Dimensional Arrays of Carbon Nanotubes,"We use numerical simulations to investigate the properties of metal contacts to three-dimensional arrays of carbon nanotubes (CNTs). For undoped arrays top-contacted with high or low work function metals, electrostatic screening is very strong, resulting in a small Schottky barrier for current injection in the top layer and large Schottky barriers for current injection in the deeper layers. As a consequence, the majority of the current flows through the top layer of the array. Our simulations show that doping of the CNT array can alleviate this problem, even without direct contact to each tube in the array; however, we find that the charge transfer length is unusually long in arrays and increases with the number of CNT layers under the contact. We also show that a bottom gate can modulate the contact resistance, but only very weakly. These results are important for the design of electronic and optoelectronic devices based on CNT arrays, because they suggest that increasing the thickness of the array does little to improve the device performance unless the film is strongly doped at the contacts and the contact is long, or unless each tube in the array is directly contacted by the metal.",1403.3942v1 2014-06-05,Giant overlap between the magnetic and superconducting phases of CeAu2Si2 under pressure,"High pressure provides a powerful means for exploring unconventional superconductivity which appears mostly on the border of magnetism. Here we report the discovery of pressure-induced heavy fermion superconductivity up to 2.5 K in the antiferromanget CeAu2Si2 (TN ~ 10 K). Remarkably, the magnetic and superconducting phases are found to overlap across an unprecedentedly wide pressure interval from 11.8 to 22.3 GPa. Moreover, both the bulk Tc and TM are strongly enhanced when increasing the pressure from 16.7 to 20.2 GPa. Tc reaches a maximum at a pressure slightly below pc ~ 22.5 GPa, at which magnetic order disappears. Furthermore, the scaling behavior of the resistivity provides evidence for a continuous delocalization of the Ce 4f-electrons associated with a critical endpoint lying just above pc. We show that the maximum Tc of CeAu2Si2 actually occurs at almost the same unit-cell volume as that of CeCu2Si2 and CeCu2Ge2, and when the Kondo and crystal field splitting energies becomes comparable. Dynamical mean-filed theory calculations suggest that the peculiar behavior in pressurized CeAu2Si2 might be related to its Ce 4f-orbital occupancy. Our results not only provide a unique example of the interplay between superconductivity and magnetism, but also underline the role of orbital physics in understanding Ce-based heavy fermion systems.",1406.1438v2 2014-09-10,Proximity effects at the interface of a superconductor and a topological insulator in NbN - Bi_2Se_3 thin film bilayers,"In a search for a simple proximity system of a topological insulator and a superconductor for studying the role of surface versus bulk effects by gating, we report here on a first step toward this goal, namely the choice of such a system and its characterization. We chose to work with thin film bilayers of grainy 5 nm thick NbN films as the superconductor, overlayed with 20 nm thick topological layer of $\rm Bi_2Se_3$ and compare the transport results to those obtained on a 5 nm thick reference NbN film on the same wafer. Bilayers with ex-situ and in-situ prepared $\rm NbN-Bi_2Se_3$ interfaces were studied and two kinds of proximity effects were found. At high temperatures just below the superconducting transition, all bilayers showed a conventional proximity effect where the topological $\rm Bi_2Se_3$ suppresses the onset or mid-transition $T_c$ of the superconducting NbN films by about 1 K. At low temperatures, a cross-over of the resistance versus temperature curves of the bilayer and reference NbN film occurs, where the bilayers show enhancement of $T_c(R=0)$, $I_c$ (the supercurrent) and the Andreev conductance, as compared to the bare NbN films. This indicates that superconductivity is induced in the $\rm Bi_2Se_3$ layer at the interface region in between the NbN grains. Thus an inverse proximity effect in the topological material is demonstrated.",1409.2975v1 2015-02-15,"Contact doping, Klein tunneling, and asymmetry of shot noise in suspended graphene","The inherent asymmetry of the electric transport in graphene is attributed to Klein tunneling across barriers defined by $\textit{pn}$-interfaces between positively and negatively charged regions. By combining conductance and shot noise experiments we determine the main characteristics of the tunneling barrier (height and slope) in a high-quality suspended sample with Au/Cr/Au contacts. We observe an asymmetric resistance $R_{\textrm{odd}}=100-70$ $\Omega$ across the Dirac point of the suspended graphene at carrier density $|n_{\rm G}|=0.3-4 \cdot 10^{11}$ cm$^{-2}$, while the Fano factor displays a non-monotonic asymmetry in the range $F_{\textrm{odd}} \sim 0.03 - 0.1$. Our findings agree with analytical calculations based on the Dirac equation with a trapezoidal barrier. Comparison between the model and the data yields the barrier height for tunneling, an estimate of the thickness of the $\textit{pn}$-interface $d < 20$ nm, and the contact region doping corresponding to a Fermi level offset of $\sim - 18$ meV. The strength of pinning of the Fermi level under the metallic contact is characterized in terms of the contact capacitance $C_c=19 \times 10^{-6}$ F/cm$^2$. Additionally, we show that the gate voltage corresponding to the Dirac point is given by the work function difference between the backgate material and graphene.",1502.04330v2 2015-10-06,Spin Hall magnetoresistance as a probe for surface magnetization in Pt/CoFe$_2$O$_4$ bilayers,"We study the spin Hall magnetoresistance (SMR) in Pt grown $\textit{in situ}$ on CoFe$_2$O$_4$ (CFO) ferrimagnetic insulating (FMI) films. A careful analysis of the angle-dependent and field-dependent longitudinal magnetoresistance indicates that the SMR contains a contribution that does not follow the bulk magnetization of CFO but it is a fingerprint of the complex magnetism at the surface of the CFO layer, thus signaling SMR as a tool for mapping surface magnetization. A systematic study of the SMR for different temperatures and CFO thicknesses gives us information impossible to obtain with any standard magnetometry technique. On one hand, surface magnetization behaves independently of the CFO thickness and does not saturate up to high fields, evidencing that the surface has its own anisotropy. On the other hand, characteristic zero-field magnetization steps are not present at the surface while they are relevant in the bulk, strongly suggesting that antiphase boundaries are the responsible of such intriguing features. In addition, a contribution from ordinary magnetoresistance of Pt is identified, which is only distinguishable due to the low resistivity of the $\textit{in-situ}$ grown Pt.",1510.01449v2 2015-11-25,Quantum oscillations of the topological surface states in low carrier concentration crystals of Bi$_{2-x}$Sb$_{x}$Te$_{3-y}$Se$_{y}$,"We report a high-field magnetotransport study on selected low-carrier crystals of the topological insulator Bi$_{2-x}$Sb${_x}$Te$_{3-y}$Se$_{y}$. Monochromatic Shubnikov - de Haas (SdH) oscillations are observed at 4.2~K and their two-dimensional nature is confirmed by tilting the magnetic field with respect to the sample surface. With help of Lifshitz-Kosevich theory, important transport parameters of the surface states are obtained, including the carrier density, cyclotron mass and mobility. For $(x,y)=(0.50,1.3)$ the Landau level plot is analyzed in terms of a model based on a topological surface state in the presence of a non-ideal linear dispersion relation and a Zeeman term with $g_s = 70$ or $-54$. Input parameters were taken from the electronic dispersion relation measured directly by angle resolved photoemission spectroscopy on crystals from the same batch. The Hall resistivity of the same crystal (thickness of 40~$\mu$m) is analyzed in a two-band model, from which we conclude that the ratio of the surface conductance to the total conductance amounts to 32~\%.",1511.08186v1 2016-05-06,Antiferromagnetism in trigonal SrMn2As2 and CaMn2As2 single crystals,"Crystallographic, electronic transport, thermal and magnetic properties are reported for SrMn2As2 and CaMn2As2 single crystals grown using Sn flux. Rietveld refinements of powder x-ray diffraction data show that the two compounds are isostructural and crystallize in the trigonal CaAl2Si2-type structure (space group P-3m1), in agreement with the literature. Electrical resistivity rho versus temperature T measurements demonstrate insulating ground states for both compounds with activation energies of 85 meV for SrMn2As2 and 61 meV for CaMn2As2. In a local-moment picture, the Mn^{+2} 3d^5 ions are expected to have high-spin S = 5/2 with spectroscopic splitting factor g = 2. Magnetic susceptibility chi and heat capacity measurements versus T reveal antiferromagnetic (AFM) transitions at TN = 120(2) K and 62(3) K for SrMn2As2 and CaMn2As2, respectively. The anisotropic chi(T < TN) data indicate that the hexagonal c axis is the hard axis and hence that the ordered Mn moments are aligned in the ab plane. The chi(T) for both compounds and Cp(T) data for SrMn2As2 show strong dynamic short-range AFM correlations from TN up to at least 900 K, likely associated with quasi-two-dimensional connectivity of strong AFM exchange interactions between the Mn spins within the corrugated honeycomb Mn layers parallel to the ab plane.",1605.02052v2 2016-06-13,Observation of Spatial Charge and Spin Correlations in the 2D Fermi-Hubbard Model,"Strong electron correlations lie at the origin of transformative phenomena such as colossal magneto-resistance and high-temperature superconductivity. Already near room temperature, doped copper oxide materials display remarkable features such as a pseudo-gap and a ""strange metal"" phase with unusual transport properties. The essence of this physics is believed to be captured by the Fermi-Hubbard model of repulsively interacting, itinerant fermions on a lattice. Here we report on the site-resolved observation of charge and spin correlations in the two-dimensional (2D) Fermi-Hubbard model realized with ultracold atoms. Antiferromagnetic spin correlations are maximal at half-filling and weaken monotonically upon doping. Correlations between singly charged sites are negative at large doping, revealing the Pauli and correlation hole\textemdash a suppressed probability of finding two fermions near each other. However, as the doping is reduced below a critical value, correlations between such local magnetic moments become positive, signaling strong bunching of doublons and holes. Excellent agreement with numerical linked-cluster expansion (NLCE) and determinantal quantum Monte Carlo (DQMC) calculations is found. Positive non-local moment correlations directly imply potential energy fluctuations due to doublon-hole pairs, which should play an important role for transport in the Fermi-Hubbard model.",1606.04089v1 2016-06-24,Epitaxial graphene homogeneity and quantum Hall effect in millimeter-scale devices,"Quantized magnetotransport is observed in 5.6 x 5.6 mm^2 epitaxial graphene devices, grown using highly constrained sublimation on the Si-face of SiC(0001) at high temperature (1900 {\deg}C). The precise quantized Hall resistance of Rxy = h/2e^2 is maintained up to record level of critical current Ixx = 0.72 mA at T = 3.1 K and 9 T in a device where Raman microscopy reveals low and homogeneous strain. Adsorption-induced molecular doping in a second device reduced the carrier concentration close to the Dirac point(n ~ 1E10 (1/cm^2)), where mobility of 43700 cm^2/Vs is measured over an area of 10 mm^2. Atomic force, confocal optical, and Raman microscopies are used to characterize the large-scale devices, and reveal improved SiC terrace topography and the structure of the graphene layer. Our results show that the structural uniformity of epitaxial graphene produced by face-to-graphite processing contributes to millimeter-scale transport homogeneity, and will prove useful for scientific and commercial applications.",1606.07720v1 2016-07-11,The electronic thermal conductivity of graphene,"Graphene, as a semimetal with the largest known thermal conductivity, is an ideal system to study the interplay between electronic and lattice contributions to thermal transport. While the total electrical and thermal conductivity have been extensively investigated, a detailed first-principles study of its electronic thermal conductivity is still missing. Here, we first characterize the electron-phonon intrinsic contribution to the electronic thermal resistivity of graphene as a function of doping using electronic and phonon dispersions and electron-phonon couplings calculated from first principles at the level of density-functional theory and many-body perturbation theory (GW). Then, we include extrinsic electron-impurity scattering using low-temperature experimental estimates. Under these conditions, we find that the in-plane electronic thermal conductivity of doped graphene is ~300 W/mK at room temperature, independently of doping. This result is much larger than expected, and comparable to the total thermal conductivity of typical metals, contributing ~10 % to the total thermal conductivity of bulk graphene. Notably, in samples whose physical or domain sizes are of the order of few micrometers or smaller, the relative contribution coming from the electronic thermal conductivity is more important than in the bulk limit, since lattice thermal conductivity is much more sensitive to sample or grain size at these scales. Last, when electron-impurity scattering effects are included, we find that the electronic thermal conductivity is reduced by 30 to 70 %. We also find that the Wiedemann-Franz law is broadly satisfied at low and high temperatures, but with the largest deviations of 20-50 % around room temperature.",1607.03037v1 2016-07-26,Interface-driven topological Hall effect in SrRuO$_3$-SrIrO$_3$ bilayer,"Electron transport coupled with magnetism has attracted attention over the years as exemplified in anomalous Hall effect due to a Berry phase in momentum space. Another type of unconventional Hall effect -- topological Hall effect, originating from the real-space Berry phase, has recently become of great importance in the context of magnetic skyrmions. We have observed topological Hall effect in bilayers consisting of ferromagnetic SrRuO$_3$ and paramagnetic SrIrO$_3$ over a wide region of both temperature and magnetic field. The topological term rapidly decreases with the thickness of SrRuO$_3$, ending up with the complete disappearance at 7 unit cells of SrRuO$_3$. Combined with model calculation, we concluded that the topological Hall effect is driven by interface Dzyaloshinskii-Moriya interaction, which is caused by both the broken inversion symmetry and the strong spin-orbit coupling of SrIrO$_3$. Such interaction is expected to realize the N\'{e}el-type magnetic skyrmion, of which size is estimated to be $\sim$10 nm from the magnitude of topological Hall resistivity. The results established that the high-quality oxide interface enables us to tune the chirality of the system; this can be a step towards the future topological electronics.",1607.07536v1 2016-08-25,Kelvin probe characterization of buried graphitic microchannels in single-crystal diamond,"In this work, we present an investigation by Kelvin Probe Microscopy (KPM) of buried graphitic microchannels fabricated in single-crystal diamond by direct MeV ion microbeam writing. Metal deposition of variable-thickness masks was adopted to implant channels with emerging endpoints and high temperature annealing was performed in order to induce the graphitization of the highly-damaged buried region. When an electrical current was flowing through the biased buried channel, the structure was clearly evidenced by KPM maps of the electrical potential of the surface region overlying the channel at increasing distances from the grounded electrode. The KPM profiling shows regions of opposite contrast located at different distances from the endpoints of the channel. This effect is attributed to the different electrical conduction properties of the surface and of the buried graphitic layer. The model adopted to interpret these KPM maps and profiles proved to be suitable for the electronic characterization of buried conductive channels, providing a non-invasive method to measure the local resistivity with a micrometer resolution. The results demonstrate the potential of the technique as a powerful diagnostic tool to monitor the functionality of all-carbon graphite/diamond devices to be fabricated by MeV ion beam lithography.",1608.07126v1 2016-08-30,"Epitaxial thin films of pyrochlore iridate Bi_{2+x}Ir_{2-y}O_{7-delta}: structure, defects and transport properties","While pyrochlore iridate thin films are theoretically predicted to possess a variety of emergent topological properties, experimental verification of these predictions can be obstructed by the challenge in thin film growth. Here we report on the pulsed laser deposition and characterization of thin films of a representative pyrochlore compound Bi2Ir2O7. The films were epitaxially grown on yttria-stabilized zirconia substrates and have lattice constants that are a few percent larger than that of the bulk single crystals. The film composition shows a strong dependence on the oxygen partial pressure. Density-functional-theory calculations indicate the existence of Bi_Ir antisite defects, qualitatively consistent with the high Bi: Ir ratio found in the films. Both Ir and Bi have oxidation states that are lower than their nominal values, suggesting the existence of oxygen deficiency. The iridate thin films show a variety of intriguing transport characteristics, including multiple charge carriers, logarithmic dependence of resistance on temperature, antilocalization corrections to conductance due to spin-orbit interactions, and linear positive magnetoresistance.",1608.08608v3 2017-10-04,"Formation, stratification, and mixing of the cores of Earth and Venus","Earth possesses a persistent, internally-generated magnetic field, whereas no trace of a dynamo has been detected on Venus, at present or in the past, although a high surface temperature and recent resurfacing events may have removed paleomagnetic evidence. Whether or not a terrestrial body can sustain an internally generated magnetic field by convection inside its metallic fluid core is determined in part by its initial thermodynamic state and its compositional structure, both of which are in turn set by the processes of accretion and differentiation. Here we show that the cores of Earth- and Venus-like planets should grow with stable compositional stratification unless disturbed by late energetic impacts. They do so because higher abundances of light elements are incorporated into the liquid metal that sinks to form the core as the temperatures and pressures of metal-silicate equilibration increase during accretion. We model this process and determine that this establishes a stable stratification that resists convection and inhibits the onset of a geodynamo. However, if a late energetic impact occurs, it could mechanically stir the core creating a single homogenous region within which a long-lasting geodynamo would operate. While Earth's accretion has been punctuated by a late giant impact with likely enough energy to mix the core (e.g. the impact that formed the Moon), we hypothesize that the accretion of Venus is characterized by the absence of such energetic giant impacts and the preservation of its primordial stratifications.",1710.01770v1 2018-03-30,Thermodynamics of Ion Separation by Electrosorption,"We present a simple, top-down approach for the calculation of minimum energy consumption of electrosorptive ion separation using variational form of the (Gibbs) free energy. We focus and expand on the case of electrostatic capacitive deionization (CDI), and the theoretical framework is independent of details of the double-layer charge distribution and is applicable to any thermodynamically consistent model, such as the Gouy-Chapman-Stern (GCS) and modified Donnan (mD) models. We demonstrate that, under certain assumptions, the minimum required electric work energy is indeed equivalent to the free energy of separation. Using the theory, we define the thermodynamic efficiency of CDI. We explore the thermodynamic efficiency of current experimental CDI systems and show that these are currently very low, less than 1% for most existing systems. We applied this knowledge and constructed and operated a CDI cell to show that judicious selection of the materials, geometry, and process parameters can be used to achieve a 9% thermodynamic efficiency (4.6 kT energy per removed ion). This relatively high value is, to our knowledge, by far the highest thermodynamic efficiency ever demonstrated for CDI. We hypothesize that efficiency can be further improved by further reduction of CDI cell series resistances and optimization of operational parameters.",1803.11532v1 2018-05-22,Non-saturating large magnetoresistance in semimetals,"The rapidly expanding class of quantum materials known as {\emph{topological semimetals}} (TSM) display unique transport properties, including a striking dependence of resistivity on applied magnetic field, that are of great interest for both scientific and technological reasons. However, experimental signatures that can identify or discern the dominant mechanism and connect to available theories are scarce. Here we present the magnetic susceptibility ($\chi$), the tangent of the Hall angle ($\tan\theta_H$) along with magnetoresistance in four different non-magnetic semimetals with high mobilities, NbP, TaP, NbSb$_2$ and TaSb$_2$, all of which exhibit non-saturating large MR. We find that the distinctly different temperature dependences, $\chi(T)$ and the values of $\tan\theta_H$ in phosphides and antimonates serve as empirical criteria to sort the MR from different origins: NbP and TaP being uncompensated semimetals with linear dispersion, in which the non-saturating magnetoresistance arises due to guiding center motion, while NbSb$_2$ and TaSb$_2$ being {\it compensated} semimetals, with a magnetoresistance emerging from nearly perfect charge compensation of two quadratic bands. Our results illustrate how a combination of magnetotransport and susceptibility measurements may be used to categorize the increasingly ubiquitous non-saturating large magnetoresistance in TSMs.",1805.08797v2 2018-09-09,Efficient thermionic operation and phonon isolation by a semiconductor-superconductor junction,"Control of heat flux at small length scales is crucial for numerous solid-state devices and systems. In addition to the thermal management of information and communication devices the mastering of heat transfer channels down to the nanoscale also enable, e.g., new memory concepts, high sensitivity detectors and sensors, energy harvesters and compact solid-state refrigerators. Electronic coolers and thermal detectors for electromagnetic radiation, especially, rely on the maximization of electro-thermal response and blockade of phonon transport. In this work, we propose and demonstrate that efficient electro-thermal operation and phonon transfer blocking can be achieved in a single solid-state thermionic junction. Our experimental demonstration relies on suspended semiconductor-superconductor junctions where the electro-thermal response arises from the superconducting energy gap, and the phonon blocking naturally results from the transmission bottleneck at the junction. We suspend different size degenerately doped silicon chips (up to macroscopic scale) directly from the junctions and cool these by biasing the junctions. The electronic cooling operation characteristics are accompanied by measurement and analysis of the thermal resistance components in the structures indicating the operation principle of phonon blocking in the junctions.",1809.02994v1 2018-11-02,Conformal printing of graphene for single and multi-layered devices on to arbitrarily shaped 3D surfaces,"Printing has drawn a lot of attention as a means of low per-unit cost and high throughput patterning of graphene inks for scaled-up thin-form factor device manufacturing. However, traditional printing processes require a flat surface and are incapable of achieving patterning on to 3D objects. Here, we present a conformal printing method to achieve functional graphene-based patterns on to arbitrarily-shaped surfaces. Using experimental design, we formulate a water-insoluble graphene ink with optimum conductivity. We then print single and multi-layered electrically functional structures on to a sacrificial layer using conventional screen printing. The print is then floated on water, allowing the dissolution of the sacrificial layer, while retaining the functional patterns. The single and multilayer patterns can then be directly transferred on to arbitrarily-shaped 3D objects without requiring any post deposition processing. Using this technique, we demonstrate conformal printing of single and multilayer functional devices that include joule heaters, resistive strain sensors and proximity sensors on hard, flexible and soft substrates, such as glass, latex, thermoplastics, textiles, and even candies and marshmallows. Our simple strategy offers great promises to add new device and sensing functionalities to previously inert 3D surfaces.",1811.01073v2 2018-11-12,Homogeneous Large-area Quasi-freestanding Monolayer and Bilayer Graphene on SiC,"In this study, we first show that the argon flow during epitaxial graphene growth is an important parameter to control the quality of the buffer and the graphene layer. Atomic force microscopy (AFM) and low-energy electron diffraction (LEED) measurements reveal that the decomposition of the SiC substrate strongly depends on the Ar mass flow rate while pressure and temperature are kept constant. Our data are interpreted by a model based on the competition of the SiC decomposition rate, controlled by the Ar flow, with a uniform graphene buffer layer formation under the equilibrium process at the SiC surface. The proper choice of a set of growth parameters allows the growth of defect-free, ultra-smooth and coherent graphene-free buffer layer and bilayer-free monolayer graphene sheets which can be transformed into large-area high-quality quasi-freestanding monolayer and bilayer graphene (QFMLG and QFBLG) by hydrogen intercalation. AFM, scanning tunneling microscopy (STM), Raman spectroscopy and electronic transport measurements underline the excellent homogeneity of the resulting quasi-freestanding layers. Electronic transport measurements in four-point probe configuration reveal a homogeneous low resistance anisotropy on both {\mu}m- and mm scales.",1811.04998v1 2018-11-14,Giant anisotropy in superconducting single crystals of CsCa$_2$Fe$_4$As$_4$F$_2$,"CsCa$_2$Fe$_4$As$_4$F$_2$ is a newly discovered iron-based superconductor with $T_\mathrm{c}\sim$ 30 K containing double Fe$_2$As$_2$ layers that are separated by insulating Ca$_2$F$_2$ spacer layers. Here we report the transport and magnetization measurements on CsCa$_2$Fe$_4$As$_4$F$_2$ single crystals grown for the first time using the self flux of CsAs. We observed a huge resistivity anisotropy $\rho_c(T)/\rho_{ab}(T)$, which increases with decreasing temperature, from 750 at 300 K to 3150 at 32 K. The $\rho_c(T)$ data exhibit a non-metallic behavior above $\sim$140 K, suggesting an incoherent electronic state at high temperatures due to the dimension crossover. The superconducting onset transition temperature in $\rho_{ab}$ is 0.7 K higher than that in $\rho_c$, suggesting two-dimensional (2D) superconducting fluctuations. The lower and upper critical fields also show an exceptional anisotropy among iron-based superconductors. The $H_{c1}^\bot(T)$ data are well fitted using the model with two $s$-wave-like superconducting gaps, $\Delta_1(0)=6.75$ meV and $\Delta_2(0)=2.32$ meV. The inter-plane coherence length $\xi_c(0)$ is $3.6$ \AA, remarkably smaller than the distance between conducting layers (8.6 \AA), consolidating the 2D nature in the title material.",1811.05706v1 2019-02-01,Light Enhanced Blue Energy Generation using MoS$_2$ Nanopores,"Blue energy relies on the chemical potential difference generated between solutions of high and low ionic strength and would provide a sun-and-wind independent energy source at estuaries around the world. Converting this osmotic energy through reverse-electrodialysis relies on ion-selective membranes. A novel generation of these membranes is based on atomically thin MoS$_2$ membranes to decrease the resistance to current flow to increase power output. By modulating the surface charge by light we are able to raise the ion selectivity of the membrane by a factor of 5 while staying at a neutral pH. Furthermore, we find that the behavior of small nanopores is dominated by surface conductance. We introduce a formalism based on the Dukhin number to quantify these effects in the case of a concentration gradient system. As a consequence, the charges created by light illumination provoke two important changes. Increased surface charge at the pore rim enhances the ion selectivity and therefore larger osmotic voltage (dominating in small pores), while the increased surface charge of the overall membrane enhances the surface conductance and therefore the osmotic current (dominating in larger pores). The combination of these effects might be able to efficiently boost the energy generation with arrays of nanopores with varying pore sizes.",1902.00410v1 2019-02-25,Synaptic Learning and Memory Functions Achieved in Self-rectifying BFO Memristor under Extreme Environmental Temperature,"Memristors have been intensively studied in recent years as promising building blocks for next-generation non-volatile memory, artificial neural networks and brain-inspired computing systems. Even though the environment adaptability of memristor has been required in many application fields, it has been rarely reported due to the underlying mechanism could become invalid especially at an elevated temperature. Here, we focus on achieving synaptic learning and memory functions in BiFeO3 memristor in a wide range of temperature. We have proved the ferroelectricity of BFO films at a record-high temperature of 500 {\deg}C by piezoresponse force microscopy (PFM) measurement. Due to the robust ferroelectricity of BFO thin film, an analog-like resistance switching behavior has been clearly found in a wide range of temperature, which is attributed to the reversal of ferroelectric polarization. Various synaptic functions including long-term potentiation (LTP), depression (LTD), consecutive potentiation/depression (P/D) and spike-timing dependent plasticity (STDP) have been realized from -170 to 300 {\deg}C, illustrating their potential for electronic applications even under extreme environmental temperature.",1902.09081v1 2019-07-03,Probing defect states in few-layer MoS$_{2}$ by conductance fluctuation spectroscopy,"Despite the concerted effort of several research groups, a detailed experimental account of defect dynamics in high-quality single- and few-layer transition metal dichalcogenides remain elusive. In this paper we report an experimental study of the temperature dependence of conductance and conductance-fluctuations on several few-layer MoS$_{2}$ exfoliated on hexagonal boron nitride and covered by a capping layer of high-$\kappa$ dielectric HfO$_{2}$. The presence of the high-$\kappa$ dielectric made the device extremely stable against environmental degradation as well as resistant to changes in device characteristics upon repeated thermal cycling enabling us to obtain reproducible data on the same device over a time-scale of more than one year. Our device architecture helped bring down the conductance fluctuations of the MoS$_2$ channel by orders of magnitude compared to previous reports. The extremely low noise levels in our devices made in possible to detect the generation-recombination noise arising from charge fluctuation between the sulphur-vacancy levels in the band gap and energy-levels at the conductance band-edge. Our work establishes conduction fluctuation spectroscopy as a viable route to quantitatively probe in-gap defect levels in low-dimensional semiconductors.",1907.01830v1 2020-04-11,High-field depinned phase and planar Hall effect in skyrmion-host Gd$_2$PdSi$_3$,"For the skyrmion-hosting intermetallic Gd$_2$PdSi$_3$ with centrosymmetric hexagonal lattice and triangular net of rare earth sites, we report a thorough investigation of the magnetic phase diagram. Our work reveals a new magnetic phase with isotropic value of the critical field for all orientations, where the magnetic ordering vector $\mathbf{q}$ is depinned from its preferred directions in the basal plane. This is in contrast to the highly anisotropic behavior of the low field phases, such as the skyrmion lattice (SkL), which are easily destroyed by in-plane magnetic field. The bulk nature of the SkL and of other magnetic phases was evidenced by specific-heat measurements. Resistivity anisotropy, likely originating from partial gapping of the density of states along $\mathbf{q}$ in this RKKY magnet, is picked up via the planar Hall effect (PHE). The PHE confirms the single-$\mathbf{q}$ nature of the magnetic order when the field is in the hexagonal plane, and allows to detect the preferred directions of $\mathbf{q}$. For field aligned perpendicular to the basal plane, several scenarios for the depinned phase (DP), such as tilted conical order, are discussed on the basis of the data.",2004.05385v1 2020-09-11,Electronic nematic states tuned by isoelectronic substitution in bulk FeSe1-xSx,"Isoelectronic substitution is an ideal tuning parameter to alter electronic states and correlations in iron-based superconductors. As this substitution takes place outside the conducting Fe planes, the electronic behaviour is less affected by the impurity scattering experimentally and relevant key electronic parameters can be accessed. In this short review, I present the experimental progress made in understanding the electronic behaviour of the nematic electronic superconductors, FeSe1-xSx. A direct signature of the nematic electronic state is in-plane anisotropic distortion of the Fermi surface triggered by orbital ordering effects and electronic interactions that result in multi-band shifts detected by ARPES. Upon sulphur substitution, the electronic correlations and the Fermi velocities decrease in the tetragonal phase. Quantum oscillations are observed for the whole series in ultra-high magnetic fields and show a complex spectra due to the presence of many small orbits. Effective masses associated to the largest orbit display non-divergent behaviour at the nematic end point (x~0.175(5)), as opposed to critical spin-fluctuations in other iron pnictides. Magnetotransport behaviour has a strong deviation from the Fermi liquid behaviour and linear T resistivity is detected at low temperatures inside the nematic phase, where scattering from low energy spin-fluctuations are likely to be present. The superconductivity is not enhanced in FeSe1-xSx and there are no divergent electronic correlations at the nematic end point. These manifestations indicate a strong coupling with the lattice in FeSe1-xSx and a pairing mechanism likely promoted by spin fluctuations.",2009.05523v1 2020-09-23,Superconducting fluctuations in overdoped Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$,"Fluctuating superconductivity - vestigial Cooper pairing in the resistive state of a material - is usually associated with low dimensionality, strong disorder or low carrier density. Here, we report single particle spectroscopic, thermodynamic and magnetic evidence for persistent superconducting fluctuations in heavily hole-doped cuprate superconductor Bi$_2$Sr$_2$CaCu$_2$O$_{8+\delta}$ ($T_c$ = 66~K) despite the high carrier density. With a sign-problem free quantum Monte Carlo calculation, we show how a partially flat band at ($\pi$,0) can help enhance superconducting phase fluctuations. Finally, we discuss the implications of an anisotropic band structure on the phase-coherence-limited superconductivity in overdoped cuprates and other superconductors.",2009.10932v2 2020-09-29,Structural Phase Dependent Giant Interfacial Spin Transparency in W/CoFeB Thin Film Heterostructure,"Pure spin current has transfigured the energy-efficient spintronic devices and it has the salient characteristic of transport of the spin angular momentum. Spin pumping is a potent method to generate pure spin current and for its increased efficiency high effective spin-mixing conductance (Geff) and interfacial spin transparency (T) are essential. Here, a giant T is reported in Sub/W(t)/Co20Fe60B20(d)/SiO2(2 nm) heterostructures in \beta-tungsten (\beta-W) phase by employing all-optical time-resolved magneto-optical Kerr effect technique. From the variation of Gilbert damping with W and CoFeB thicknesses, the spin diffusion length of W and spin-mixing conductances are extracted. Subsequently, T is derived as 0.81 \pm 0.03 for the \beta-W/CoFeB interface. A sharp variation of Geff and T with W thickness is observed in consonance with the thickness-dependent structural phase transition and resistivity of W. The spin memory loss and two-magnon scattering effects are found to have negligible contributions to damping modulation as opposed to spin pumping effect which is reconfirmed from the invariance of damping with Cu spacer layer thickness inserted between W and CoFeB. The observation of giant interfacial spin transparency and its strong dependence on crystal structures of W will be important for pure spin current based spin-orbitronic devices.",2009.14143v1 2017-04-20,Accretion powered AGN feedback in the cores of galaxy clusters,"Detection of the copious amount of X-ray emission from the dilute hot plasma in galaxy clusters suggests that a substantial fraction of the central intracluster medium (ICM) is cooling radiatively on a time scale much faster than the Hubble time. Theoretical models predict the cooling rate as high as about few hundred to few thousand solar mass per year, which would be then made available for the formation of new stars in the core of these clusters. However, systematic studies of the cores of such clusters failed to detect the expected reservoirs of cooled gas. Thus, the gas in the cores of galaxy clusters is losing substantial amount of energy in the form of X-rays but is not cooling. This in turn point towards the famous cooling flow paradox and hence demands some intermittent heating to balance the cooling over such a long period. Several sources have been suggested to counteract on the cooling of the ICM, however, the AGN feedback appeared to be the most promising and enough energetic source to resist cooling of the ICM in the cores of such clusters. In this presentation I will provide a brief overview on the feedback processes that are involved in the cores of the galaxy clusters with an emphasis on the AGN feedback and its observable signatures.",1704.06047v1 2017-04-23,Steep-slope Hysteresis-free Negative Capacitance MoS2 Transistors,"The so-called Boltzmann Tyranny defines the fundamental thermionic limit of the subthreshold slope (SS) of a metal-oxide-semiconductor field-effect transistor (MOSFET) at 60 mV/dec at room temperature and, therefore, precludes the lowering of the supply voltage and the overall power consumption. Adding a ferroelectric negative capacitor to the gate stack of a MOSFET may offer a promising solution to bypassing this fundamental barrier. Meanwhile, two-dimensional (2D) semiconductors, such as atomically thin transition metal dichalcogenides (TMDs) due to their low dielectric constant, and ease of integration in a junctionless transistor topology, offer enhanced electrostatic control of the channel. Here, we combine these two advantages and demonstrate for the first time a molybdenum disulfide (MoS2) 2D steep slope transistor with a ferroelectric hafnium zirconium oxide layer (HZO) in the gate dielectric stack. This device exhibits excellent performance in both on- and off-states, with maximum drain current of 510 {\mu}A/{\mu}m, sub-thermionic subthreshold slope and is essentially hysteresis-free. Negative differential resistance (NDR) was observed at room temperature in the MoS2 negative capacitance field-effect-transistors (NC-FETs) as the result of negative capacitance due to the negative drain-induced-barrier-lowering (DIBL). High on-current induced self-heating effect was also observed and studied.",1704.06865v2 2017-08-04,The cuprate phase diagram and the influence of nanoscale inhomogeneities,"The phase diagram associated with the high Tc superconductors is complicated by an array of different ground states. The parent material represents an antiferromagnetic insulator but with doping superconductivity becomes possible with transition temperatures previously thought unattainable. The underdoped region of the phase diagram is dominated by the so-called pseudogap phenomena whereby in the normal state the system mimics superconductivity in its spectra response but does not show the complete loss of resistivity associated with the superconducting state. An understanding of this regime presents one of the great challenges for the field. In the present study we revisit the structure of the phase diagram as determined in photoemission studies. By careful analysis of the role of nanoscale inhomogeneities in the overdoped region we are able to more carefully separate out the gaps due to the pseudogap phenomena from the gaps due to the superconducting transition. Within a mean field description we are thus able to link the magnitude of the gap directly to the Heisenberg exchange interaction term, $J\sum{s_i \cdot s_j}$, contained in the $t-J$ model. This approach provides a clear indication that the pseudogap is that associated with spin singlet formation.",1708.01558v2 2019-03-12,Precision Analysis of Evolved Stars,"Evolved stars dominate galactic spectra, enrich the galactic medium, expand to change their planetary systems, eject winds of a complex nature, produce spectacular nebulae and illuminate them, and transfer material between binary companions. While doing this, they fill the HR diagram with diagnostic loops that write the story of late stellar evolution. Evolved stars sometimes release unfathomable amounts of energy in neutrinos, light, kinetic flow, and gravitational waves. During these late-life times, stars evolve complexly, with expansion, convection, mixing, pulsation, mass loss. Some processes have virtually no spatial symmetries, and are poorly addressed with low-resolution measurements and analysis. Even a ""simple"" question as how to model mass loss resists solution. However, new methods offer increasingly diagnostic tools. Astrometry reveals populations and groupings. Pulsations/oscillations support study of stellar interiors. Optical/radio interferometry enable 2-3d imagery of atmospheres and shells. Bright stars with rich molecular spectra and velocity fields are a ripe opportunity for imaging with high spatial and spectral resolution, giving insight into the physics and modeling of later stellar evolution.",1903.05109v1 2019-04-14,Superconducting Praseodymium Superhydrides,"Superhydrides have complex hydrogenic sublattices and are important prototypes for studying metallic hydrogen and high-temperature superconductors. Encouraged by the results on LaH10, in consideration of the differences between La and Pr, Pr-H system is especially worth studying because of the magnetism and valence-band f-electrons in element Pr. Here we successfully synthesized praseodymium superhydrides (PrH9) in laser-heated diamond anvil cells. Synchrotron X-ray diffraction (XRD) analysis demonstrated the presence of previously predicted F43m-PrH9 and unexpected P63/mmc-PrH9 phases. Moreover, Fm3m-PrH3, P4/nmm-PrH(3-{\delta}) and Fm3m-PrH(1+x) were found below 52 GPa. F43m-PrH9 and P63/mmc-PrH9 were stable above 100 GPa in experiment. Experimental studies of electrical resistance in the PrH9 sample showed the emergence of superconducting transition (Tc) below 9K and a dependent Tc on applied magnetic field. Theoretical calculations indicate that magnetic order and electron-phonon interaction coexist in a very close range of pressures in the PrH9 sample which may contribute to its low superconducting temperature Tc. Our results highlight the intimate connections among hydrogenic sublattices, density of states, magnetism and superconductivity in Pr-based superhydrides.",1904.06643v2 2019-08-06,Hump-like structure in Hall signal from SrRuO$_3$ ultra-thin films without inhomogeneous anomalous Hall effect,"A controversy arose over the interpretation of the recently observed hump features in Hall resistivity $\rho_{xy}$ from ultra-thin SrRuO$_3$ (SRO) film; it was initially interpreted to be due to topological Hall effect but was later proposed to be from existence of regions with different anomalous Hall effect (AHE). In order to settle down the issue, we performed Hall effect as well as magneto-optic Kerr-effect measurements on 4 unit cell SRO films grown on SrTiO$_3$ (001) substrates. Clear hump features are observed in the measured $\rho_{xy}$, whereas neither hump feature nor double hysteresis loop is seen in the Kerr rotation which should be proportional to the magnetization. In addition, magnetization measurement by superconducting quantum interference device shows no sign of multiple coercive fields. These results show that inhomogeneous AHE alone cannot explain the observed hump behavior in $\rho_{xy}$ data from our SRO ultra-thin films. We found that emergence of the hump structure in $\rho_{xy}$ is closely related to the growth condition, high quality films having clear sign of humps.",1908.02083v1 2019-08-22,High-Pressure Synthesis of Magnetic Neodymium Polyhydrides,"The current search for room-temperature superconductivity is inspired by the unique properties of the electron-phonon interaction in metal superhydrides. Encouraged by the recently found highest-$T_C$ superconductor fcc-$LaH_{10}$, here we discover several superhydrides of another lanthanide - neodymium. We identify three novel metallic Nd-H phases at pressure range from 85 to 135 GPa: $I4/mmm$-$NdH_4$, $C2/c$-$NdH_7$, $P6_3/mmc$-$NdH_9$, synthesized by laser-heating metal samples in NH3BH3 media for in situ generation of hydrogen. A lower trihydride $Fm\bar{3}m$-$NdH_3$ is found at pressures from 2 to 52 GPa. $I4/mmm$-$NdH_4$ and $C2/c$-$NdH_7$ are stable from 135 down to 85 GPa, and $P6_3/mmc$-$NdH_9$ from 110 to 130 GPa. Measurements of the electrical resistance of NdH9 demonstrate a possible superconducting transition at ~4.5 K in $P6_3/mmc$-$NdH_9$. Our theoretical calculations predict that all the neodymium hydrides have antiferromagnetic order at pressures below 150 GPa and represent one of the first discovered examples of strongly correlated superhydrides with large exchange spin-splitting in the electron band structure (> 450 meV). The critical N$\'e$el temperatures for new neodymium hydrides are estimated using the mean-field approximation as about 4 K ($NdH_4$), 251 K ($NdH_7$) and 136 K ($NdH_9$).",1908.08304v3 2019-12-27,Localized spin waves at low temperatures in a Cobalt Carbide nanocomposite,"We study magnetic, transport and thermal properties of Cobalt carbide nanocomposite with a mixture of Co2C and Co3C phases in 1:1 ratio, with an average particle diameter of 40$\pm 15$ nm. We show that the behavior of the nanocomposite is completely different from that of either Co3C or Co2C. We observed that with decreasing temperature the saturation magnetization MS(T) increases, however, below 100 K, there is a steep rise. A detail analysis shows the increase in MS(T) down to 100 K is explained via the surface spin freezing model. However, below 100 K the steep increase in MS(T) is explained by a finite size effect related to a confinement of spin waves within the nano particles. The measurement of heat capacity shows broad peak at 100 K along with presence of another anomaly at a lower temperature 43 K(=Tex). Resistance measurement in the nanocomposite shows metallic behavior at high T with an unusual anomaly appearing at Tex, which is near the T regime where MS(T) begins to increase steeply. A measurement of the temperature gradients across the sample thickness indicates an abrupt change in thermal conductivity at Tex which suggests a phase transition at Tex. Our results are explained in terms of a transformation from a magnetically coupled state with a continuous spectrum of spin waves into a magnetically decoupled state below 100 K with confined spin waves.",1912.12085v1 2012-06-06,Irreversibility and time relaxation in electrostatic doping of oxide interfaces,"Two-dimensional electron gas (2DEG) confined in quantum wells at insulating oxide interfaces have attracted much attention as their electronic properties display a rich physics with various electronics orders such as superconductivity and magnetism. A particularly exciting features of these hetero-structures lies in the possibility to control their electronic properties by electrostatic gating, opening up new opportunities for the development of oxide based electronics. However, unexplained gating hysteresis and time relaxation of the 2DEG resistivity have been reported in some bias range, raising the question of the precise role of the gate voltage. Here we show that in LaTiO3/SrTiO3 and LaAlO3/SrTiO3 heterostructures, above a filling threshold, electrons irreversibly escape out of the well. This mechanism, which is directly responsible for the hysteresis and time relaxation, can be entirely described by a simple analytical model derived in this letter. Our results highlight the crucial role of the gate voltage both on the shape and the filling of the quantum well. They also demonstrate that it is possible to achieve a low-carrier density regime in a semiconductor limit, whereas the high-carrier density regime is intrinsically limited.",1206.1198v1 2018-07-04,Doping effects of Cr on the physical properties of BaFe$_{1.9-x}$Ni$_{0.1}$Cr$_{x}$As$_{2}$,"We present a systematic study on the heavily Cr doped iron pnictides BaFe$_{1.9-x}$Ni$_{0.1}$Cr$_{x}$As$_{2}$ by using elastic neutron scattering, high-resolution synchrotron X-ray diffraction (XRD), resistivity and Hall transport measurements. When the Cr concentration increases from $x=$ 0 to 0.8, neutron diffraction experiments suggest that the collinear antiferromagnetism persists in the whole doping range, where the N\'{e}el temperature $T_N$ coincides with the tetragonal-to-orthorhombic structural transition temperature $T_s$, and both of them keeps around 35 K. The magnetic ordered moment, on the other hand, increases within increasing $x$ until $x=$ 0.5, and then decreases with further increasing $x$. Detailed refinement of the powder XRD patterns reveals that the Cr substitutions actually stretch the FeAs$_4$ tetrahedron along the $c-$axis and lift the arsenic height away Fe-Fe plane. Transport results indicate that the charge carriers become more localized upon Cr doping, then changes from electron-type to hole-type around $x=$ 0.5. Our results suggest that the ordered moment and the ordered temperature of static magnetism in iron pnictides can be decoupled and tuned separately by chemical doping.",1807.01612v1 2018-07-26,Excitation and coherent control of spin qudit modes with sub-MHz spectral resolution,"Quantum bit or qubit is a two-level system, which builds the foundation for quantum computation, simulation, communication and sensing. Quantum states of higher dimension, i.e., qutrits (D = 3) and especially qudits (D = 4 or higher), offer significant advantages. Particularly, they can provide noise-resistant quantum cryptography, simplify quantum logic and improve quantum metrology. Flying and solid-state qudits have been implemented on the basis of photonic chips and superconducting circuits, respectively. However, there is still a lack of room-temperature qudits with long coherence time and high spectral resolution. The silicon vacancy centers in silicon carbide (SiC) with spin S = 3/2 are quite promising in this respect, but until now they were treated as a canonical qubit system. Here, we apply a two-frequency protocol to excite and image multiple qudit modes in a SiC spin ensemble under ambient conditions. Strikingly, their spectral width is about one order of magnitude narrower than the inhomogeneous broadening of the corresponding spin resonance. By applying Ramsey interferometry to these spin qudits, we achieve a spectral selectivity of 600 kHz and a spectral resolution of 30 kHz. As a practical consequence, we demonstrate absolute DC magnetometry insensitive to thermal noise and strain fluctuations.",1807.10383v1 2018-12-16,Anti-fatigue-fracture hydrogels,"The emerging applications of hydrogels in devices and machines require these soft materials to maintain robustness under cyclic mechanical loads. Whereas hydrogels have been made tough to resist fracture under a single cycle of mechanical load, these toughened gels still suffer from fatigue fracture under multiple cycles of loads. The reported fatigue threshold (i.e., the minimal fracture energy at which crack propagation occurs under cyclic loads) for synthetic hydrogels is on the order of 1-100 J/m2, which is primarily associated with the energy required to fracture a single layer of polymer chains per unit area. Here, we demonstrate that the controlled introduction of crystallinity in hydrogels can significantly enhance their fatigue thresholds, since the process of fracturing crystalline domains for fatigue-crack propagation requires much higher energy than fracturing a single layer of polymer chains. The fatigue threshold of polyvinyl alcohol (PVA) with a crystallinity of 18.9 wt.% in the swollen state can exceed 1,000 J/m2. We further develop a strategy to enhance the anti-fatigue-fracture properties of PVA hydrogels, but still maintain their high water contents and low moduli by patterning highly-crystalline regions in the hydrogels. The current work not only reveals an anti-fatigue-fracture mechanism in hydrogels but also provides a practical method to design anti-fatigue-fracture hydrogels for diverse applications.",1812.06403v1 2019-01-15,Use of Cernox thermometers in AC specific heat measurements under pressure,"We report on the resistance behavior of bare-chip Cernox thermometers under pressures up to 2 GPa, generated in a piston-cylinder pressure cell. Our results clearly show that Cernox thermometers, frequently used in low-temperature experiments due to their high sensitivity, remain highly sensitive even under applied pressure. We show that these thermometers are therefore ideally suited for measurements of heat capacity under pressure utilizing an ac oscillation technique up to at least 150 K. Our Cernox-based system is very accurate in determining changes of the specific heat as a function of pressure as demonstrated by measurements of the heat capacity on three different test cases: (i) the superconducting transition in elemental Pb (T_{c} = 7.2 K), (ii) the antiferromagnetic transition in the rare-earth compound GdNiGe3 (T_{N} = 26 K) and (iii) the structural/magnetic transition in the iron-pnictide BaFe2As2 (T_{s,N} = 130 K). The chosen examples demonstrate the versatility of our technique for measuring the specific heat under pressure of various condensed matter systems with very different transition temperatures as well as amounts of removed entropy.",1901.05089v2 2019-10-07,High electrical conductivity of single metal-organic chains,"Molecular wires are essential components for future nanoscale electronics. However, the preparation of individual long conductive molecules is still a challenge. MMX metal-organic polymers are quasi-one-dimensional sequences of single halide atoms (X) bridging subunits with two metal ions (MM) connected by organic ligands. They are excellent electrical conductors as bulk macroscopic crystals and as nanoribbons. However, according to theoretical calculations, the electrical conductance found in the experiments should be even higher. Here we demonstrate a novel and simple drop-casting procedure to isolate bundles of few to single MMX chains. Furthermore, we report an exponential dependence of the electrical resistance of one or two MMX chains as a function of their length that does not agree with predictions based on their theoretical band structure. We attribute this dependence to strong Anderson localization originated by structural defects. Theoretical modeling confirms that the current is limited by structural defects, mainly vacancies of iodine atoms, through which the current is constrained to flow. Nevertheless, measurable electrical transport along distances beyond 250 nm surpasses that of all other molecular wires reported so far. This work places in perspective the role of defects in one-dimensional wires and their importance for molecular electronics.",1910.02834v1 2020-10-01,Universal limiting transition temperature for the high $T_\mathrm{c}$ superconductors,"Since their discovery three decades ago it has emerged that the physics of high-$T_\mathrm{c}$ cuprate superconductors is characterised by multiple temperature scales, and a phenomenology that deviates significantly from the conventional paradigm of superconductivity. Below the ""pseudogap"" temperature, $T^*$, a range of experiments indicate a reduction in the density of states. Lower in temperature, $T_\mathrm{c}$ marks the onset of a bulk zero-resistance state. Intermediate between these, numerous other temperature boundaries and cross-overs have been identified, often postulated to be associated with fluctuations of some kind. However, for the most part there is little consensus either over their definitions or the physical mechanisms at play. One of these temperature scales is the Nernst onset temperature, $T_\mathrm{onset}$, below which thermoelectric phenomena characteristic of superconductivity are observed. Depending on the material, the difference between $T_\mathrm{onset}$ and $T_\mathrm{c}$ ranges from almost nothing to over 100K. In this paper, we identify $T_\mathrm{onset}$ from published experimental data according to a consistent definition; this reveals a remarkable consistency of behaviour across the whole high-$T_\mathrm{c}$ family, despite the appreciable variations in other parameters. Our analysis suggests that in the cuprates there is an inherent limit to $T_\mathrm{c} \sim 135$K. We compare this behaviour with other strongly-correlated superconductors and propose a unified picture of superconducting fluctuations close to the Mott state.",2010.00572v1 2020-11-17,Shallow Valence Band of Rutile GeO$_2$ and P-type Doping,"GeO$_2$ has an $\alpha$-quartz-type crystal structure with a very wide fundamental band gap of 6.6 eV and is a good insulator. Here we find that the stable rutile-GeO$_2$ polymorph with a 4.6 eV band gap has a surprisingly low $\sim$6.8 eV ionization potential, as predicted from the band alignment using first-principles calculations. Because of the short O$-$O distances in the rutile structure containing cations of small effective ionic radii such as Ge$^{4+}$, the antibonding interaction between O 2p orbitals raises the valence band maximum energy level to an extent that hole doping appears feasible. Experimentally, we report the flux growth of $1.5 \times 1.0 \times 0.8$ mm$^3$ large rutile GeO$_2$ single crystals and confirm the thermal stability for temperatures up to $1021 \pm 10~^\circ$C. X-ray fluorescence spectroscopy shows the inclusion of unintentional Mo impurities from the Li$_2$O$-$MoO$_3$ flux, as well as the solubility of Ga in the r-GeO$_2$ lattice as a prospective acceptor dopant. The resistance of the Ga- and Mo-codoped r-GeO$_2$ single crystals is very high at room temperature, but it decreases by 2-3 orders of magnitude upon heating to 300 $^\circ$C, which is attributed to thermally-activated p-type conduction.",2011.08928v1 2020-11-25,Evidence for freezing of charge degrees of freedom across a critical point in CeCoIn$_5$,"The presence of a quantum critical point separating two distinct zero-temperature phases is thought to underlie the `strange' metal state of many high-temperature superconductors. The nature of this quantum critical point, as well as a description of the resulting strange metal, are central open problems in condensed matter physics. In large part, the controversy stems from the lack of a clear broken symmetry to characterize the critical phase transition, and this challenge is no clearer than in the example of the unconventional superconductor CeCoIn$_5$. Through Hall effect and Fermi surface measurements of CeCoIn$_5$, in comparison to ab initio calculations, we find evidence for a critical point that connects two Fermi surfaces with different volumes without apparent symmetry-breaking, indicating the presence of a transition that involves an abrupt localization of one sector of the charge degrees of freedom. We present a model for the anomalous electrical Hall resistivity of this material based on the conductivity of valence charge fluctuations.",2011.12951v1 2020-12-03,Effect of ageing on the properties of the W-containing IRIS-TiAl alloy,"The effects of ageing at 800 $^\circ$C on the properties of the IRIS alloy (Ti$_{49.9}$Al$_{48}$W$_2$B$_{0.1}$) are studied. The initial microstructure of this alloy densified by Spark Plasma Sintering (SPS) is mainly composed of lamellar colonies which are surrounded by $\gamma$ grains. The evolutions of the alloy strength and creep resistance resulting from this ageing treatment are measured by the related mechanical tests. The microstructural changes are investigated by scanning and transmission electron microscopies and by X-ray diffraction. The main structural evolutions consist in a shrinkage of the lamellar areas and in a precipitation of $\beta_0$ phase, which is accompanied by a moderate segregation of tungsten and a decrease of the $\alpha_2$ lamellar width. However, these evolutions are relatively limited and the microstructural stability is found to result mainly from the low diffusivity of tungsten. Conversely, a moderate effect of this ageing treatment on mechanical properties, at room and high temperatures, is measured. Such experimental results are interpreted and discussed in terms of the microstructural evolutions and of the deformation mechanisms which are activated at different temperatures under various solicitations.",2012.01760v1 2020-12-03,First order transition in trigonal structure ${\textbf{Ca}}{\textbf{Mn}}_{2}{\textbf{P}}_{2}$,"We report structural and physical properties of the single crystalline ${\mathrm{Ca}}{\mathrm{Mn}}_{2}{\mathrm{P}}_{2}$. The X-ray diffraction(XRD) results show that ${\mathrm{Ca}}{\mathrm{Mn}}_{2}{\mathrm{P}}_{2}$ adopts the trigonal ${\mathrm{Ca}}{\mathrm{Al}}_{2}{\mathrm{Si}}_{2}$-type structure. Temperature dependent electrical resistivity $\rho(T)$ measurements indicate an insulating ground state for ${\mathrm{Ca}}{\mathrm{Mn}}_{2}{\mathrm{P}}_{2}$ with activation energies of 40 meV and 0.64 meV for two distinct regions, respectively. Magnetization measurements show no apparent magnetic phase transition under 400 K. Different from other ${\mathrm{A}}{\mathrm{Mn}}_{2}{\mathrm{Pn}}_{2}$ (A = Ca, Sr, and Ba, and Pn = P, As, and Sb) compounds with the same structure, heat capacity $C_{\mathrm{p}}(T)$ and $\rho(T)$ reveal that ${\mathrm{Ca}}{\mathrm{Mn}}_{2}{\mathrm{P}}_{2}$ has a first-order transition at $T$ = 69.5 K and the transition temperature shifts to high temperature upon increasing pressure. The emergence of plenty of new Raman modes below the transition, clearly suggests a change in symmetry accompanying the transition. The combination of the structural, transport, thermal and magnetic measurements, points to an unusual origin of the transition.",2012.01863v1 2021-02-10,Electropolishing of single crystal and polycrystalline aluminum to achieve high optical and mechanical surfaces,"Electropolishing has found wide application as the final surface treatment of metal products in mechanical engineering and instrumentation, medicine and reflective concentrators for PV cells. It was found that electropolishing (EP) not only reduces the surface roughness and changes its appearance, but improves many operational characteristics as well, such as corrosion resistance, endurance, tensile strength, and many others, and also changes the physicochemical properties, for example, reflectivity, electromagnetic permeability and electronic emission of some ferro-magnetic metals. This fact greatly expands the possibility of using this method in various fields of science and technology. This work is part of a study, examining electro polishing for reducing the crystalline defects adjacent to the surface, thus improving its physical properties, contributing to higher optical efficiency, when used in PV generation and storage devices. Five compositions were examined using different temperature and current density parameters. The polished samples were evaluated using reflectance spectrometry. The solution which was composed of Phosphoric acid - 85%, Acetic acid - 10%, Nitric acid - 5% was found to provide the best results. Another result obtained was that reflectance increased as the current density increased up to 25 A/dm2. Further increasing the current density resulted in deterioration of the surface and reduced reflectance. It was shown that careful lapping and polishing followed by electropolishing using the suggested solution may consist of an adequate treatment for preparing reflective concentrators for PV cells.",2102.05752v1 2021-04-21,Electrically driven programmable phase-change meta-switch reaching 80% efficiency,"Despite recent advances in active metaoptics, wide dynamic range combined with high-speed reconfigurable solutions is still elusive. Phase-change materials (PCMs) offer a compelling platform for metasurface optical elements, owing to the large index contrast and fast yet stable phase transition properties. Here, we experimentally demonstrate an in situ electrically-driven reprogrammable metasurface by harnessing the unique properties of a phase-change chalcogenide alloy, Ge$_{2}$Sb$_{2}$Te$_{5}$ (GST), in order to realize fast, non-volatile, reversible, multilevel, and pronounced optical modulation in the near-infrared spectral range. Co-optimized through a multiphysics analysis, we integrate an efficient heterostructure resistive microheater that indirectly heats and transforms the embedded GST film without compromising the optical performance of the metasurface even after several reversible phase transitions. A hybrid plasmonic-PCM meta-switch with a record electrical modulation of the reflectance over eleven-fold (an absolute reflectance contrast reaching 80%), unprecedented quasi-continuous spectral tuning over 250 nm, and switching speed that can potentially reach a few kHz is presented. Our work represents a significant step towards the development of fully integrable dynamic metasurfaces and their potential for beamforming applications.",2104.10381v2 2021-07-01,Solid Source Metal-Organic Molecular Beam Epitaxy of Epitaxial RuO2,"A seemingly simple oxide with a rutile structure, RuO2 has been shown to possess several intriguing properties ranging from strain-stabilized superconductivity to a strong catalytic activity. Much interest has arisen surrounding the controlled synthesis of RuO2 films but, unfortunately, utilizing atomically-controlled deposition techniques like molecular beam epitaxy (MBE) has been difficult due to the ultra-low vapor pressure and low oxidation potential of Ru. Here, we demonstrate the growth of epitaxial, single-crystalline RuO2 films on different substrate orientations using the novel solid-source metal-organic (MO) MBE. This approach circumvents these issues by supplying Ru using a pre-oxidized solid metal-organic precursor containing Ru. High-quality epitaxial RuO2 films with bulk-like room-temperature resistivity of 55 micro-ohm-cm were obtained at a substrate temperature as low as 300 C. By combining X-ray diffraction, transmission electron microscopy, and electrical measurements, we discuss the effect of substrate temperature, orientation, film thickness, and strain on the structure and electrical properties of these films. Our results illustrating the use of novel solid-source MOMBE approach paves the way to the atomic-layer controlled synthesis of complex oxides of stubborn metals, which are not only difficult to evaporate but also hard to oxidize.",2107.00193v1 2021-08-02,PID-like active control strategy for electroacoustic resonators to design tunable single-degree-of-freedom sound absorbers,"Sound absorption at low frequencies still remains a challenge in both scientific research and engineering practice. Natural porous materials are ineffective in this frequency range, as well as acoustic resonators which present too narrow bandwidth of absorption, thus requiring alternative solutions based on active absorption techniques. In the present work, we propose an active control framework applied on a closed-box loudspeaker to enable the adjustment of the acoustic impedance at the loudspeaker diaphragm. More specifically, based on the proportionality between the pressure inside the enclosure and the axial displacement of the loudspeaker diaphragm at low frequencies, we demonstrate both analytically and experimentally that a PID-like feedback control approach allows tuning independently the compliance, the resistance and the moving mass of the closed-box loudspeaker to implement a prescribed impedance of a single-degree-of-freedom resonator. By considering different control combinations to tailor the resonator characteristics, a perfect absorption (with absorption coefficient equal to 1) is achievable at the target resonance frequency, while enlarging the effective absorption bandwidth. Moreover, the proposed feedback control strategy shows an excellent control accuracy, especially compared to the feedforward-based control formerly reported in the literature. The mismatches between the performance of experimental prototype and the model, likely to result from the control time delay and the inaccuracy in estimating the loudspeaker parameters, can be compensated directly by tuning the control parameters in the control platform. The active resonators implemented through the reported control scheme can be used to build more complex acoustic devices/structures to enable high-efficiency broadband sound absorption or other types of acoustic phenomena such as wavefront shaping.",2108.00765v1 2021-10-29,Supercurrent diode effect and magnetochiral anisotropy in few-layer NbSe$_2$,"Nonreciprocal transport refers to charge transfer processes that are sensitive to the bias polarity. Until recently, nonreciprocal transport was studied only in dissipative systems, where the nonreciprocal quantity is the resistance. Recent experiments have, however, demonstrated nonreciprocal supercurrent leading to the observation of a supercurrent diode effect in Rashba superconductors, opening the vision of dissipationless electronics. Here we report on a supercurrent diode effect in NbSe$_2$ constrictions obtained by patterning NbSe$_2$ flakes with both even and odd layer number. The observed rectification is driven by valley-Zeeman spin-orbit interaction. We demonstrate a rectification efficiency as large as 60%, considerably larger than the efficiency of devices based on Rashba superconductors. In agreement with recent theory for superconducting transition metal dichalcogenides, we show that the effect is driven by an out-of-plane magnetic field component. Remarkably, we find that the effect becomes field-asymmetric in the presence of an additional in-plane field component transverse to the current direction. Supercurrent diodes offer a further degree of freedom in designing superconducting quantum electronics with the high degree of integrability offered by van der Waals materials.",2110.15752v2 2021-11-28,CoFeVSb: A Promising Candidate for Spin Valve and Thermoelectric Applications,"We report a combined theoretical and experimental study of a novel quaternary Heusler system CoFeVSb from the view point of room temperature spintronics and thermoelectric applications. It crystallizes in cubic structure with small DO$_3$-type disorder. The presence of disorder is confirmed by room temperature synchrotron X-ray diffraction(XRD) and extended X-ray absorption fine structure (EXAFS) measurements. Magnetization data reveal high ordering temperature with a saturation magnetization of 2.2 $\mu_B$/f.u. Resistivity measurements reflect half-metallic nature. Double hysteresis loop along with asymmetry in the magnetoresistance(MR) data reveals room temperature spin-valve feature, which remains stable even at 300 K. Hall measurements show anomalous behavior with significant contribution from intrinsic Berry phase. This compound also large room temperature power factor ($\sim0.62$ mWatt/m/K$^{2}$) and ultra low lattice thermal conductivity ($\sim0.4$ W/m/K), making it a promising candidate for thermoelectric application. Ab-initio calculations suggest weak half-metallic behavior and reduced magnetization (in agreement with experiment) in presence of DO$_3$ disorder. We have also found an energetically competing ferromagnetic FM)/antiferromagnetic (AFM) interface structure within an otherwise FM matrix: one of the prerequisites for spin valve behavior. Coexistence of so many promising features in a single system is rare, and hence CoFeVSb gives a fertile platform to explore numerous applications in future.",2111.14081v1 2021-12-16,Constrained multi-objective optimization of process design parameters in settings with scarce data: an application to adhesive bonding,"Adhesive joints are increasingly used in industry for a wide variety of applications because of their favorable characteristics such as high strength-to-weight ratio, design flexibility, limited stress concentrations, planar force transfer, good damage tolerance, and fatigue resistance. Finding the optimal process parameters for an adhesive bonding process is challenging: the optimization is inherently multi-objective (aiming to maximize break strength while minimizing cost), constrained (the process should not result in any visual damage to the materials, and stress tests should not result in failures that are adhesion-related), and uncertain (testing the same process parameters several times may lead to different break strengths). Real-life physical experiments in the lab are expensive to perform. Traditional evolutionary approaches (such as genetic algorithms) are then ill-suited to solve the problem, due to the prohibitive amount of experiments required for evaluation. Although Bayesian optimization-based algorithms are preferred to solve such expensive problems, few methods consider the optimization of more than one (noisy) objective and several constraints at the same time. In this research, we successfully applied specific machine learning techniques (Gaussian Process Regression) to emulate the objective and constraint functions based on a limited amount of experimental data. The techniques are embedded in a Bayesian optimization algorithm, which succeeds in detecting Pareto-optimal process settings in a highly efficient way (i.e., requiring a limited number of physical experiments).",2112.08760v3 2022-01-08,Are Heavy Fermion Strange Metals Planckian?,"Strange metal behavior refers to a linear temperature dependence of the electrical resistivity at temperatures below the Mott-Ioffe-Regel limit. It is seen in numerous strongly correlated electron systems, from the heavy fermion compounds, via transition metal oxides and iron pnictides, to magic angle twisted bi-layer graphene, frequently in connection with unconventional or ""high temperature"" superconductivity. To achieve a unified understanding of these phenomena across the different materials classes is a central open problem in condensed matter physics. Tests whether the linear-in-temperature law might be dictated by Planckian dissipation - scattering with the rate $\sim k_{\rm B}T/\hbar$, are receiving considerable attention. Here we assess the situation for strange metal heavy fermion compounds. They allow to probe the regime of extreme correlation strength, with effective mass or Fermi velocity renormalizations in excess of three orders of magnitude. Adopting the same procedure as done in previous studies, i.e., assuming a simple Drude conductivity with the above scattering rate, we find that for these strongly renormalized quasiparticles, scattering is much weaker than Planckian, implying that the linear temperature dependence should be due to other effects. We discuss implications of this finding and point to directions for further work.",2201.02820v1 2022-03-04,"Character of the ""normal state"" of the nickelate superconductors","The occurrence of superconductivity in proximity to various strongly correlated phases of matter has drawn extensive focus on their normal state properties, to develop an understanding of the state from which superconductivity emerges. The recent finding of superconductivity in layered nickelates raises similar interests. However, transport measurements of doped infinite-layer nickelate thin films have been hampered by materials limitations of these metastable compounds - in particular, a relatively high density of extended defects. Here, by moving to a substrate (LaAlO$_{3}$)$_{0.3}$(Sr$_{2}$TaAlO$_{6}$)$_{0.7}$ which better stabilizes the growth and reduction conditions, we can synthesize the doping series of Nd$_{1-x}$Sr$_{x}$NiO$_{2}$ essentially free from extended defects. This enables the first examination of the 'intrinsic' temperature and doping dependent evolution of the transport properties. The normal state resistivity exhibits a low-temperature upturn in the underdoped regime, linear behavior near optimal doping, and quadratic temperature dependence for overdoping. This is strikingly similar to the copper oxides, despite key distinctions - namely the absence of an insulating parent compound, multiband electronic structure, and a Mott-Hubbard orbital alignment rather than the charge-transfer insulator of the copper oxides. These results suggest an underlying universality in the emergent electronic properties of both superconducting families.",2203.02580v1 2022-03-22,Prediction of resistance induced by surface complexity in lubricating layers: Application to super-hydrophobic surfaces,"Super Hydrophobic (SH) coatings are widely used to mitigate drag in various applications. Numerous studies have demonstrated that the beneficial wall-slip effect produced by these materials disappears in laminar flow regimes. The main mechanisms considered to be behind the decrease in performance are Marangoni-induced stresses and air/liquid interface deformation. In the present study, a new mechanism is proposed to explain the loss of performances of SH-surfaces in laminar flow regimes. Here we consider the flow of air inside the plastron and the associated momentum loses induced by roughness elements with different geometric characteristics. The effects of air motion within the plastron is coupled to the outer fluid with a homogenised boundary condition approach. To this end, numerical simulations at the scale of the roughness element were conducted as a function of the porosity and the tortuosity of the domain to determine the slip velocity at the air-liquid interface. The homogenised boundary condition is then implemented in a theoretical model for the outer flow to compute drag on SH-spheres at low $Re$ numbers. Experiments of laminar SH falling spheres indicate that high values of the tortuosity and low values of porosity lead to a loss of performances when considering drag reduction. As anticipated, a 3D printed sphere with low tortuosity and similar porosity demonstrated near-optimal drag reductions. A comparative study between the predicted values and experiments shows that the homogenised model is able to accurately predict the drag on SH surfaces for values of the porosity and tortuosity estimated from microscopy images of the SH textured surface.",2203.12039v1 2022-04-06,Thermal activation of low-density Ga implanted in Ge,"The nuclear spins of low-density implanted Ga atoms in Ge are interesting candidates for solid state-based qubits. To date, activation studies of implanted Ga in Ge have focused on high densities. Here we extend activation studies into the low-density regime. We use spreading resistance profiling and secondary ion mass spectrometry to derive electrical activation of Ga ions implanted into Ge as a function of rapid thermal anneal temperature and implant density. We show that for our implant conditions the activation is best for anneal temperatures between 400 and 650 $^\circ$C, with a maximum activation of 64% at the highest fluence. Below 400 $^\circ$C, remaining implant damage results in defects that act as superfluous carriers, and above 650 $^\circ$C, surface roughening and loss of Ga ions are observed. The activation increased monotonically from 10% to 64% as the implant fluence increased from $6\times10^{10}$ to $6\times10^{12}$ cm$^{-2}$. The results provide thermal anneal conditions to be used for initial studies of using low-density Ga atoms in Ge as nuclear spin qubits.",2204.02878v1 2022-05-05,Intrinsic spin Hall torque in a moire Chern magnet,"In spin torque magnetic memories, electrically actuated spin currents are used to switch a magnetic bit. Typically, these require a multilayer geometry including both a free ferromagnetic layer and a second layer providing spin injection. For example, spin may be injected by a nonmagnetic layer exhibiting a large spin Hall effect, a phenomenon known as spin-orbit torque. Here, we demonstrate a spin-orbit torque magnetic bit in a single two-dimensional system with intrinsic magnetism and strong Berry curvature. We study AB-stacked MoTe2/WSe2, which hosts a magnetic Chern insulator at a carrier density of one hole per moire superlattice site. We observe hysteretic switching of the resistivity as a function of applied current. Magnetic imaging using a superconducting quantum interference device reveals that current switches correspond to reversals of individual magnetic domains. The real space pattern of domain reversals aligns precisely with spin accumulation measured near the high-Berry curvature Hubbard band edges. This suggests that intrinsic spin- or valley-Hall torques drive the observed current-driven magnetic switching in both MoTe2/WSe2 and other moire materials. The switching current density of 10^3 Amps per square centimeter is significantly less than reported in other platforms paving the way for efficient control of magnetic order.",2205.02823v1 2022-06-02,A multi-fidelity approach coupling parameter space reduction and non-intrusive POD with application to structural optimization of passenger ship hulls,"Nowadays, the shipbuilding industry is facing a radical change towards solutions with a smaller environmental impact. This can be achieved with low emissions engines, optimized shape designs with lower wave resistance and noise generation, and by reducing the metal raw materials used during the manufacturing. This work focuses on the last aspect by presenting a complete structural optimization pipeline for modern passenger ship hulls which exploits advanced model order reduction techniques to reduce the dimensionality of both input parameters and outputs of interest. We introduce a novel approach which incorporates parameter space reduction through active subspaces into the proper orthogonal decomposition with interpolation method. This is done in a multi-fidelity setting. We test the whole framework on a simplified model of a midship section and on the full model of a passenger ship, controlled by 20 and 16 parameters, respectively. We present a comprehensive error analysis and show the capabilities and usefulness of the methods especially during the preliminary design phase, finding new unconsidered designs while handling high dimensional parameterizations.",2206.01243v3 2022-06-08,Dielectric properties and impedance spectroscopy of NASICON type Na$_3$Zr$_2$Si$_2$PO$_{12}$,"We report the temperature dependent dielectric properties and impedance spectroscopy investigation of Na$_3$Zr$_2$Si$_2$PO$_{12}$ in the frequency range of 20 Hz--2 MHz. The Rietveld refinement of x-ray diffraction pattern confirms the monoclinic phase with C2/c space group. The {\it d.c.} resistivity behavior shows its strong insulating nature at low temperatures, and follows Arrhenius law of thermal conduction with an activation energy of 0.68 eV. The decrease in electric permittivity ($\epsilon_r$) with frequency is explained based on the space polarization mechanism and its increment with temperature by thermal activation of charge carriers. The dielectric loss (D=tan$\delta$) peak follows the Arrhenius law of thermal activation with an energy of 0.25 eV. We observe an enhancement in {\it a.c.} conductivity with frequency and temperature due to the decrease in the activation energy, which results in enhancing the conduction between defect states. Further, we observe an abrupt increase in the {\it a.c.} conductivity at high frequencies, which is explained using the universal Jonschers power law. The analysis of {\it a.c.} conductivity shows two types of conduction mechanisms namely correlated barrier hopping and non-overlapping small polaron tunnelling in the measured temperature range. The imaginary part of the electric modulus confirms the non-Debye type relaxation in the sample. The shifting of the relaxation peak towards higher frequency side with an increase in temperature ensures its thermally activated nature. The scaling behavior of the electric modulus shows similar type of relaxation over the measured temperature range. The combined analysis of electric modulus and impedance with frequency shows the short-range mobility of charge carriers.",2206.03668v1 2022-11-18,Synthesis of infinite-layer nickelates and influence of the capping-layer on magnetotransport,"The recent discovery of a zero-resistance state in nickel-based compounds has generated a re-excitement about the long-standing problem in condensed matter of high-critical-temperature superconductivity, in light of the analogies between infinite-layer nickelates and cuprates. However, despite some formal valence and crystal symmetry analogies, the electronic properties of infinite-layer nickelates are remarkably original accounting, among other properties, of a unique Nd5d-Ni3d hybridization. This designates infinite-layer nickelates as a new class of oxide superconductors which should be considered on their own. Here we report about Nd1-xSrxNiO2 (x = 0, 0.05 and 0.2) thin films synthesized with and without a SrTiO3 capping-layer, showing very smooth and step-terraced surface morphologies. Angle-dependent anisotropic magnetoresistance measurements performed with a magnetic field rotating in-plane or out-of-plane with respect to the sample surface, rendered important information about the magnetic properties of undoped SrTiO3-capped and uncapped samples. The results point at a key role of the capping-layer in controlling the magnitude and the anisotropy of the anisotropic magnetoresistance properties. We discuss this control in terms of a combined effect between the Nd-Ni hybridization and an intra-atomic exchange coupling between the Nd-4f and Nd-5d states, the latter essentially contributing to the (magneto)transport. Further studies foresee the influence of the capping layer on infinite-layer nickelates with no magnetic rare-earth.",2211.10251v1 2022-12-12,Unconventional localization of electrons inside of a nematic electronic phase,"The magnetotransport behaviour inside the nematic phase of bulk FeSe reveals unusual multiband effects that cannot be reconciled with a simple two-band approximation proposed by surface-sensitive spectroscopic probes. In order to understand the role played by the multiband electronic structure and the degree of two-dimensionality we have investigated the electronic properties of exfoliated flakes of FeSe by reducing their thickness. Based on magnetotransport and Hall resistivity measurements, we assess the mobility spectrum that suggests an unusual asymmetry between the mobilities of the electrons and holes with the electron carriers becoming localized inside the nematic phase. Quantum oscillations in magnetic fields up to 38 T indicate the presence of a hole-like quasiparticle with a lighter effective mass and a quantum scattering time three times shorter, as compared with bulk FeSe. The observed localization of negative charge carriers by reducing dimensionality can be driven by orbitally-dependent correlation effects, enhanced interband spin-fluctuations or a Lifshitz-like transition which affect mainly the electron bands. The electronic localization leads to a fragile two-dimensional superconductivity in thin flakes of FeSe, in contrast to the two-dimensional high-Tc induced with electron doping via dosing or using a suitable interface.",2212.06196v1 2023-01-19,Ab initio comparison of spin-transport properties in MgO-spaced ferrimagnetic tunnel junctions based on Mn$_3$Ga and Mn$_3$Al,"We report on first-principles spin-polarised quantum transport calculations (from NEGF+DFT) in MgO-spaced magnetic tunnel junctions (MTJs) based on two different Mn-based Heusler ferrimagnetic metals, namely Mn$_3$Al and Mn$_3$Ga in their tetragonal DO$_{22}$ phase. The former is a fully compensated half-metallic ferrimagnet, while the latter is a low-moment high-spin-polarisation ferrimagnet, both with a small lattice mismatch from MgO. In identical symmetric and asymmetric interface reconstructions across a 3-monolayer thick MgO barrier for both ferrimagets, the linear response (low-voltage) spin-transfer torque (STT) and tunneling magneto-resistance (TMR) effects are evaluated. A larger staggered in-plane STT is found in the Mn$_3$Ga case, while the STT in Mn$_3$Al vanishes quickly away from the interface (similarly to STT in ferromagnetic MTJs). The roles are reversed for the TMR, which is practically 100\% in the half-metallic Mn$_3$Al-based MTJs (using the conservative definition) as opposed to 60\% in the Mn$_3$Ga case. The weak dependence on the exact interface reconstruction would suggest Mn$_3$Ga-Mn$_3$Al solid solutions as a possible route towards optimal trade-off of STT and TMR in the low-bias, low-temperature transport regime.",2301.08300v1 2023-05-09,Influence of Shape on Heteroaggregation of Model Microplastics: A Simulation Study,"Nano- and microplastics are a growing threat for the environment, especially in aqueous habitats. For assessing the influence on the ecosystem and possible solution strategies, it is necessary to investigate the fate of microplastics (MP) in the environment. MPs are typically surrounded by natural organic matter, which can cause them to aggregate. However, the effect of MP shape and flow conditions on this heteroaggregation is not well understood. To address this gap, we perform simulations of heteroaggregation of different MP shapes with smaller spherical organic matter. We demonstrate that the shape had a strong impact on the aggregate structure. MPs with mostly smooth surfaces formed compact structures with a large number of neighbors with weak connection strength and a higher fractal dimension. MPs with edges and corners aggregated into more fractal structures with fewer neighbors, but with stronger connections. Using MPCD, we investigated aggregates under shear flow. The critical shear rate at which the aggregates break up is much larger for spherical and rounded cube MPs, i.e, the compact aggregate structure of spheres outweighs their weaker connection strength. Most notably, the rounded cube exhibited unexpectedly high resistance against breakup under shear. We attribute this to being fairly compact due to weaker, flexible neighbor connections, which are still strong enough to prevent particles to break off during shear flow. Irrespective of the stronger connections between neighbouring MPs, the fractal aggregates of cubes break up at lower shear rates. We find that cube aggregates reduced their radius of gyration significantly, indicating restructuring, while most neighbor connections were kept intact. Aggregates of spheres, however, kept their overall size while undergoing local rearrangements, that broke a significant portion of their neighbor interactions.",2305.05453v1 2023-06-08,Epitaxial thin films of binary Eu-compounds close to a valence transition,"Intermetallic binary compounds of europium reveal a variety of interesting phenomena due to the interconnection between two different magnetic and 4f electronic (valence) states, which are particularly close in energy. The valence states or magnetic properties are thus particularly sensitive to strain-tuning in these materials. Consequently, we grew epitaxial EuPd$_2$ (magnetic Eu$^{2+}$) and EuPd$_3$ (nonmagnetic Eu$^{3+}$) thin films on MgO(001) substrates using molecular beam epitaxy. Ambient X-ray diffraction confirms an epitaxial relationship of cubic Laves-type (C15) EuPd$_2$ with an (111)-out-of-plane orientation, whereby eight distinct in-plane crystallographic domains develop. For simple cubic EuPd$_3$ two different out-of-plane orientations can be obtained by changing the substrate annealing temperature under ultra-high vacuum conditions from 600 {\deg}C to 1000 {\deg}C for one hour. A small resistance minimum evolves for EuPd$_3$ thin films grown with low temperature substrate annealing, which was previously found even in single crystals of EuPd$_3$ and might be attributed to a Kondo or weak localization effect. Absence of influence of an applied magnetic fields and magnetotransport measurements suggest a nonmagnetic ground state for EuPd$_3$ thin films, i. e., a purely trivalent Eu valence, as found in EuPd$_3$ single crystals. For EuPd$_2$ magnetic ordering below ~72 K is observed, quite similar to single crystal behavior. Field dependent measurements of the magnetoresistance and the Hall effect show hysteresis effects below ~0.4 T and an anomalous Hall effect below ~70 K, which saturates around 1.4 T, thus proving a ferromagnetic ground state of the divalent Eu.",2306.05355v2 2023-06-26,Phase purity and surface morphology of high-Jc superconducting Bi2Sr2Ca1Cu2O8+δ thin films,"Bi2Sr2Ca1Cu2O8+d (Bi-2212) thin films with thicknesses less than 50 nm (<20 unit cells) are grown by pulsed laser deposition (PLD) onto (001) LaAlO3 (LAO) single crystal substrates. Phase-pure and smooth c-axis oriented Bi-2212 films with optimal oxygen doping, critical temperature Tc0 up to 86 K, and critical current density Jc(60 K) above 1 MA/cm2 are obtained for samples that are annealed in situ at temperatures below 700 {\deg}C. At higher temperature Bi-2212 films on LAO substrates partially decompose to non-superconducting impurity phases, while films on MgO and SrTiO3 substrates are stable. The broadening of Tc of the metal-to-superconductor resistive phase transition in magnetic fields is much larger for thin films of Bi-2212 as compared to YBa2Cu3O7. The magnetic field-induced suppression of Tc0 is stronger for Bi-2212 films containing impurity phases as compared to the phase-pure Bi-2212 films. The degradation of LAO substrate crystals after several steps of deposition and chemical removal of the Bi-2212 layer is investigated. New, commercially prepared substrates provide Bi-2212 films with smallest surface roughness (3 nm) and strong out-of-plane texture. However, thin films of almost the same quality are obtained on re-used LAO substrates that are mechanically polished after the chemical etching.",2306.14481v1 2023-07-12,Coexistence of Competing Microbial Strains under Twofold Environmental Variability and Demographic Fluctuations,"Microbial populations generally evolve in volatile environments, under conditions fluctuating between harsh and mild, e.g. as the result of sudden changes in toxin concentration or nutrient abundance. Environmental variability thus shapes the long-time population dynamics, notably by influencing the ability of different strains of microorganisms to coexist. Inspired by the evolution of antimicrobial resistance, we study the dynamics of a community consisting of two competing strains subject to twofold environmental variability. The level of toxin varies in time, favouring the growth of one strain under low drug concentration and the other strain when the toxin level is high. We also model time-changing resource abundance by a randomly switching carrying capacity that drives the fluctuating size of the community. While one strain dominates in a static environment, we show that species coexistence is possible in the presence of environmental variability. By computational and analytical means, we determine the environmental conditions under which long-lived coexistence is possible and when it is almost certain. Notably, we study the circumstances under which environmental and demographic fluctuations promote, or hinder, the strains coexistence. We also determine how the make-up of the coexistence phase and the average abundance of each strain depend on the environmental variability.",2307.06314v3 2023-07-31,Synthesis of possible room temperature superconductor LK-99:Pb$_9$Cu(PO$_4$)$_6$O,"The quest for room-temperature superconductors has been teasing scientists and physicists, since its inception in 1911 itself. Several assertions have already been made about room temperature superconductivity but were never verified or reproduced across the labs. The cuprates were the earliest high transition temperature superconductors, and it seems that copper has done the magic once again. Last week, a Korean group synthesized a Lead Apatite-based compound LK-99, showing a T$_c$ of above 400$^\circ$K. The signatures of superconductivity in the compound are very promising, in terms of resistivity (R = 0) and diamagnetism at T$_c$. Although, the heat capacity (C$_p$) did not show the obvious transition at T$_c$. Inspired by the interesting claims of above room temperature superconductivity in LK-99, in this article, we report the synthesis of polycrystalline samples of LK-99, by following the same heat treatment as reported in [1,2] by the two-step precursor method. The phase is confirmed through X-ray diffraction (XRD) measurements, performed after each heat treatment. The room temperature diamagnetism is not evidenced by the levitation of a permanent magnet over the sample or vice versa. Further measurements for the confirmation of bulk superconductivity on variously synthesized samples are underway. Our results on the present LK-99 sample, being synthesized at 925$^\circ$C, as of now do not approve the appearance of bulk superconductivity at room temperature. Further studies with different heat treatments are though, yet underway.",2307.16402v2 2023-10-11,Temperature-Dependent Collective Excitations in a Three-Dimensional Dirac System ZrTe$_{5}$,"Zirconium pentatelluride (ZrTe$_{5}$), a system with a Dirac linear band across the Fermi level and anomalous transport features, has attracted considerable research interest for it is predicted to be located at the boundary between strong and weak topological insulators separated by a topological semimetal phase. However, the experimental verification of the topological phase transition and the topological ground state in ZrTe$_{5}$ is full of controversies, mostly due to the difficulty of precisely capturing the small gap evolution with single-particle band structure measurements. Alternatively, the collective excitations of electric charges, known as plasmons, in Dirac systems exhibiting unique behavior, can well reflect the topological nature of the band structure. Here, using reflective high-resolution electron energy loss spectroscopy (HREELS), we investigate the temperature-dependent collective excitations of ZrTe$_{5}$, and discover that the plasmon energy in ZrTe$_{5}$ is proportional to the $1/3$ power of the carrier density $n$, which is a unique feature of plasmons in three-dimensional Dirac systems. Based on this conclusion, the origin of the resistivity anomaly of ZrTe$_{5}$ can be attributed to the temperature-dependent chemical potential shift in extrinsic Dirac semimetals.",2310.07232v2 2023-10-19,"Comparison of the Resistivities of Nanostructured Films Made from Silver, Copper-Silver and Copper Nanoparticle and Nanowire Suspensions","Spray deposition and inkjet printing of various nanostructures are emerging complementary methods for creating conductive coatings on different substrates. In comparison to established deposition techniques like vacuum metal coating and lithography-based metallization processes, spray deposition and inkjet printing benefit from significantly simplified equipment. However, there are number of challenges related to peculiar properties and behaviour of nanostructures that require additional studies. In present work, we investigate electroconductive properties and sintering behaviour of thin films produced from nanostructures of different metals (Ag, Cu and Cu-Ag) and different shapes (nanowires and spherical nanoparticles), and compare them to the reference Ag and Cu magnetron deposited films. Synthesized nanostructures were studied with transmission electron microscopy. Morphology and crystallinity of produced metal films were studied with scanning electron microscopy and X-ray diffraction. The electrical parameters were measured by the van der Pauw method. All nanowires-based films provided high conductivity and required only modest thermal treatment (200 C). To achieve sufficient sintering and conductivity of nanoparticles-based films, higher temperatures are required (300 C for Ag nanoparticles and 350 C for Cu and Cu-Ag nanoparticles). Additionally, stability of nanowires was studied by annealing the samples in vacuum conditions inside a scanning electron microscope at 500 C.",2310.12506v1 2023-11-01,Active Noise Control Portable Device Design,"While our world is filled with its own natural sounds that we can't resist enjoying, it is also chock-full of other sounds that can be irritating, this is noise. Noise not only influences the working efficiency but also the human's health. The problem of reducing noise is one of great importance and great difficulty. The problem has been addressed in many ways over the years. The current methods for noise reducing mostly rely on the materials and transmission medium, which are only effective to some extent for the high frequency noise. However, the effective reduction noise method especially for low frequency noise is very limited. Here we come up with a noise reduction system consist of a sensor to detect the noise in the environment. Then the noise will be sent to an electronic control system to process the noise, which will generate a reverse phase frequency signal to counteract the disturbance. Finally, the processed smaller noise will be broadcasted by the speaker. Through this smart noise reduction system, even the noise with low-frequency can be eliminated. The system is also integrated with sleep tracking and music player applications. It can also remember and store settings for the same environment, sense temperature, and smart control of home furniture, fire alarm, etc. This smart system can transfer data easily by Wi-Fi or Bluetooth and controlled by its APP. In this project, we will present a model of the above technology which can be used in various environments to prevent noise pollution and provide a solution to the people who have difficulties finding a peaceful and quiet environment for sleep, work or study.",2311.00535v1 2023-11-13,Superconductivity in trilayer nickelate La4Ni3O10 under pressure,"Nickelate superconductors have attracted a great deal of attention over the past few decades due to their similar crystal and electronic structures with high-temperature cuprate superconductors. Here, we report the superconductivity in a pressurized Ruddlesden-Popper phase single crystal, La4Ni3O10 (n = 3), and its interplay with the density wave order in the phase diagram. With increasing pressure, the density wave order as indicated by the anomaly in the resistivity is progressively suppressed, followed by the emergence of the superconductivity around 25 K. Our angle-resolved photoemission spectroscopy measurements reveal that the electronic structure of La4Ni3O10 is very similar to that of La3Ni2O7, suggesting unified electronic properties of nickelates in Ruddlesden-Popper phases. Moreover, theoretical analysis unveils that antiferromagnetic (AFM) super-exchange interactions can serve as the effective pairing interaction for the emergence of superconductivity (SC) in pressurized La4Ni3O10. Our research provides a new platform for the investigation of the unconventional superconductivity mechanism in Ruddlesden-Popper trilayer perovskite nickelates.",2311.07423v2 2023-11-15,Quantification of cell contractile behavior based on non-destructive macroscopic measurement of tension forces on bioprinted hydrogel,"Contraction assay based on surface measurement have been widely used to evaluate cell contractility in 3D models. This method is straightforward and requires no specific equipment, but it does not provide quantitative data about contraction forces generated by cells. We expanded this method with a new biomechanical model, based on the work-energy theorem, to provide non-destructive longitudinal monitoring of contraction forces generated by cells in 3D.We applied this method on hydrogels seeded with either fibroblasts or osteoblasts. Hydrogel mechanical characteristics were modulated to enhance (condition HCA$_{High}$: hydrogel contraction assay high contraction) or limit (condition HCA$_{Low}$: hydrogel contraction assay low contraction) cell contractile behaviors. Macroscopic measures were further correlated with cell contractile behavior and descriptive analysis of their physiology in response to different mechanical environments. Fibroblasts and osteoblasts contracted their matrix up to 47% and 77% respectively. Contraction stress peaked at day 5 with 1.1 10$^{-14}$Pa for fibroblasts and 3.5 10$^{-14}$Pa for osteoblasts, which correlated with cell attachment and spreading. Negligible contraction was seen in HCA$_{Low}$. Both fibroblasts and osteoblasts expressed $\alpha$-SMA contractile fibers in HCA$_{High}$ and HCA$_{Low}$. Failure to contract HCA$_{Low}$ was attributed to increased cross-linking and resistance to proteolytic degradation of the hydrogel.",2311.08773v1 2023-12-15,Plasma-enhanced atomic layer deposition of titanium nitride for superconducting devices,"This study presents a comprehensive investigation into the exceptional superconducting attributes of titanium nitride (TiN) achieved through plasma-enhanced atomic layer deposition (PEALD) on both planar and intricate three-dimensional (3D) structures. We introduced an additional substrate biasing cycle to densify the film and remove ligand residues, augmenting the properties while minimizing impurities. While reactive-sputtered TiN films exhibit high quality, our technique ensures superior uniformity by consistently maintaining a desired sheet resistance greater than 95 percent across a 6inch wafer, a critical aspect for fabricating extensive arrays of superconducting devices and optimizing wafer yield. Moreover, our films demonstrate exceptional similarity to conventional reactive-sputtered films, consistently reaching a critical temperature (Tc) of 4.35 K with a thickness of around 40 nm. This marks a notable achievement compared to previously reported ALD-based superconducting TiN. Using the same process as for planar films, we obtained Tc for aspect ratios (ARs) ranging from 2 to 40, observing a Tc of approximately 2 K for ARs between 2 and 10.5. We elucidate the mechanisms contributing to the limitations and degradation of superconducting properties over these aggressive 3D structures. Our results seamlessly align with both current and next-generation superconducting technologies, meeting stringent criteria for thin-film constraints, large-scale deposition, conformality, 3D integration schemes, and yield optimization.",2312.09984v1 2023-12-19,On the role of Grain Boundary Character in the Stress Corrosion Cracking of Nanoporous Gold Thin Films,"For its potential as a catalyst, nanoporous gold (NPG) prepared through dealloying of bulk Ag-Au alloys has been extensively investigated. NPG thin films can offer ease of handling, better tunability of the chemistry and microstructure of the nanoporous structure, and represent a more sustainable usage of scarce resources. These films are however prone to intergranular cracking during dealloying, limiting their stability and potential applications. Here, we set out to systematically investigate the grain boundaries in Au28Ag72 thin films. We observe that a sample synthesized at 400 {\deg}C is at least 2.5 times less prone to cracking compared to a sample synthesized at room temperature. This correlates with a higher density of coincident site lattice grain boundaries, especially the density of coherent sigma 3, increased, which appear resistant against cracking. Nanoscale compositional analysis of random high-angle grain boundaries reveals prominent Ag enrichment up to 77 at.%, whereas sigma 3 coherent twin boundaries show Au enrichment of up to 30 at.%. The misorientation and the chemistry of grain boundaries hence affect their dealloying behavior, which in turn controls the cracking, and the possible longevity of NPG thin films for application in electrocatalysis.",2312.12235v1 2024-02-26,Electronic phase transitions and superconductivity in ferroelectric Sn$_2$P$_2$Se$_6$ under pressure,"Since there is both strong electron-phonon coupling during a ferroelectric/FE transition and superconducting/SC transition, it has been an important topic to explore superconductivity from the FE instability. Sn$_2$P$_2$Se$_6$ arouses broad attention due to its unique FE properties. Here, we reported the electronic phase transitions and superconductivity in this compound based on high-pressure electrical transport measurement, optical absorption spectroscopy and Raman based structural analysis. Upon compression, the conductivity of Sn$_2$P$_2$Se$_6$ was elevated monotonously, an electronic phase transition occurred near 5.4 GPa, revealed by optical absorption spectroscopy, and the insulating state is estimated to be fully suppressed near 15 GPa. Then, it started to show the signature of superconductivity near 15.3 GPa. The zero-resistance state was presented from 19.4 GPa, and the superconductivity was enhanced with pressure continuously. The magnetic field effect further confirmed the SC behavior and this compound had a $T_c$ of 5.4 K at 41.8 GPa with a zero temperature upper critical field of 6.55 T. The Raman spectra confirmed the structural origin of the electronic transition near 5.4 GPa, which should due to the transition from the paraelectric phase to the incommensurate phase, and suggested a possible first-order phase transition when the sample underwent the semiconductor-metal transition near 15 GPa. This work demonstrates the versatile physical properties in ferroelectrics and inspires the further investigation on the correlation between FE instability and SC in M$_2$P$_2$X$_6$ family.",2402.16427v1 2024-02-29,Anomalous frequency and temperature dependent scattering in the dilute metallic phase in lightly doped-SrTiO$_3$,"The mechanism of superconductivity in materials with aborted ferroelectricity and the emergence of a dilute metallic phase in systems like doped-SrTiO$_3$ are outstanding issues in condensed matter physics. This dilute metal has features both similar and different to those found in the normal state of other unconventional superconductors. We have investigated the optical properties of the dilute metallic phase in doped-SrTiO$_3$ using THz time-domain spectroscopy. At low frequencies the THz response exhibits a Drude-like form as expected for typical metal-like conductivity. We observed the frequency and temperature dependencies to the low energy scattering rate $\Gamma(\omega, T) \propto (\hbar\omega)^2 + (p \pi k_BT)^2 $ expected in a conventional Fermi liquid, despite the fact that densities are too small to allow current decay through electron-electron scattering. However we find the lowest known $p$ values of 0.39-0.72. As $p$ is 2 in a canonical Fermi liquid and existing models based on energy dependent elastic scattering bound $p$ from below to 1, our observation lies outside current explanation. Our data also gives insight into the high temperature regime and shows that the temperature dependence of the resistivity derives in part from strong T dependent mass renormalizations.",2402.18767v1 2024-03-06,"Crystal, ferromagnetism, and magnetoresistance with sign reversal in a EuAgP semiconductor","We synthesized the ferromagnetic EuAgP semiconductor and conducted a comprehensive study of its crystalline, magnetic, heat capacity, band gap, and magnetoresistance properties. Our investigation utilized a combination of X-ray diffraction, optical, and PPMS DynaCool measurements. EuAgP adopts a hexagonal structure with the $P6_3/mmc$ space group. As the temperature decreases, it undergoes a magnetic phase transition from high-temperature paramagnetism to low-temperature ferromagnetism. We determined the ferromagnetic transition temperature to be $T_{\textrm{C}} =$ 16.45(1) K by fitting the measured magnetic susceptibility using a Curie-Weiss law. Heat capacity analysis of EuAgP considered contributions from electrons, phonons, and magnons, revealing $\eta$ = 0.03 J/mol/$\textrm{K}^\textrm{2}$, indicative of semiconducting behavior. Additionally, we calculated a band gap of $\sim$ 1.324(4) eV based on absorption spectrum measurements. The resistivity versus temperature of EuAgP measured in the absence of an applied magnetic field shows a pronounced peak around $T_{\textrm{C}}$, which diminishes rapidly with increasing applied magnetic fields, ranging from 1 to 14 T. An intriguing phenomenon emerges in the form of a distinct magnetoresistance transition, shifting from positive (e.g., 1.95\% at 300 K and 14 T) to negative (e.g., -30.73\% at 14.25 K and 14 T) as the temperature decreases. This behavior could be attributed to spin-disordered scattering.",2403.03650v1 2024-03-20,Optimizing Transparent Electrodes: Interplay of High Purity SWCNTs network and a Polymer,"The discovery of transparent electrodes led to the development of optoelectronic devices such as OLEDs, LCDs, touchscreens, IR sensors, etc. Since ITO has many drawbacks in respect of its production cost and limited transparency in IR, carbon nanotubes (CNTs) have been a potential replacement for ITO due to their exceptional electrical and optical properties, especially in the IR region. In this work, we present the development of a CNT-polymer composite thin film that exhibits outstanding transparency across both visible and IR spectra prepared by layer-by-layer (LbL) technique. This approach not only ensures uniform integration and crosslinking of CNTs into lightweight matrices, but also represents a cost-effective method for producing transparent electrodes with remarkable optical and electrical properties. The produced films achieved a transparency above 80% in the UV-VIS range and approximately 70% in the mid-IR range. The sheet resistance of the fabricated thin films was measured at about 4 kOhm/sq, showing a tendency to decrease with the number of bilayers. Furthermore, in this work we have investigated electrical properties and transport mechanisms in more detail with computational analysis. Computational analysis was performed to better understand the electrical behavior of nanotube-polymer junctions in the interbundle structure. Based on all results, we propose that the transparent electrodes with 4 and 6 bilayers are the most optimal structures in terms of optical and electrical properties.",2403.13594v1 1996-10-01,Itinerant Antiferromagnetism in FeGe_2,"FeGe_2, and lightly doped compounds based on it, have a Fermi surface driven instability which drive them into an incommensurate spin density wave state. Studies of the temperature and magnetic field dependence of the resistivity have been used to determine the magnetic phase diagram of the pure material which displays an incommensurate phase at high temperatures and a commensurate structure below 263 K in zero field. Application of a magnetic field in the tetragonal basal plane decreases the range of temperatures over which the incommensurate phase is stable. We have used inelastic neutron scattering to measure the spin dynamics of FeGe_2. Despite the relatively isotropic transport the magnetic dynamics is quasi-one dimensional in nature. Measurements carried out on HET at ISIS have been used to map out the spin wave dispersion along the c-axis up the 400 meV, more than an order of magnitude higher than the zone boundary magnon for wavevectors in the basal plane.",9610009v1 1998-05-25,Metal-insulator transition induced by 16O -18O oxygen isotope exchange in colossal negative magnetoresistance manganites,"The effect of 16O-18O isotope exchange on the electric resistivity was studied for (La(1-y)Pr(y))0.7Ca0.3MnO3 ceramic samples. Depending on y, this mixed perovskite exhibited different types of low-temperature behavior ranging from ferromagnetic metal (FM) to charge ordered (CO) antiferromagnetic insulator. It was found that at y=0.75, the substitution of 16O by 18O results in the reversible transition from a FM to a CO insulator at zero magnetic field. The applied magnetic field (H >= 2 T) transformed the sample with 18O again to the metallic state and caused the increase in the FM transition temperature Tc of the 16O sample. As a result, the isotope shift of Tc at H = 2 T was as high as 63 K. Such unique sensitivity of the system to oxygen isotope exchange, giving rise even to the metal-insulator transition, is discussed in terms of the isotope dependence of the effective electron bandwidth which shifts the balance between the CO and FM phases.",9805315v1 2001-04-13,Metal-insulator transition in 2D: a role of the upper Habbard band,"To explain the main features of the metal-insulator transition (MIT) in 2D we suggest a simple model taking into account strongly localized states in the band tail of 2D conductivity band with a specific emphasize of a role of doubly-occupied states (upper Hubbard band). The metallic behavior of resistance is explained as result of activation of localized electrons to conductance band leading to a suppression of non-linear screening of the disorder potential. The magnetoresistance (MR) in the critical region is related to depopulation of double occupied localized states also leading to partial suppression of the nonlinear screening. The most informative data are related to nearly activated temperature dependence of MR in strongly insulating limit (which can be in particular reached from the metallic state in high enough fields). According to our model this behavior originates due to a lowering of a position of chemical potential in the upper Hubbard band due to Zeeman splitting. We compare the theoretical predictions to the existing experimental data and demonstrate that the model explains such features of the 2D MIT as scaling behavior in the critical region, saturation of MR and H/T scaling of MR in the insulating limit. The quantitative analysis of MR in strongly insulating limit based on the model suggested leads to the values of g-factors being in good agreement with known values for localized states in corresponding materials.",0104254v1 2001-05-31,Anomalous Nonlinear Microwave Response of Epitaxial YBa2Cu3O7-x Films on MgO,"We have investigated the anomalous nonlinear microwave response of epitaxial electron-beam coevaporated YBa2Cu3O7-x films on MgO. The power and temperature dependent surface impedance and two-tone intermodulation distortion were measured in stripline resonators at several frequencies between 2.3 and 11.2 GHz and at temperatures between 1.7 K and Tc. All of the eight films measured to date show a decrease of the surface resistance Rs of up to one order of magnitude as the microwave current is increased up to approximately 1 mA for T < 20 K. The surface reactance Xs showed only a weak increase in the same region. The usual nonlinear increase of Rs and Xs was observed at high currents in the 100-mA range. The minimum of Rs correlates with a pronounced plateau in the third-order intermodulation signal. We have developed a phenomenological two-fluid model, incorporating a microwave current-dependent quasiparticle scattering rate g and normal fraction fn. The model contains only three adjustable parameters. We find good agreement with the measured data for constant fn and a current-dependent scattering rate g whose magnitude increases almost linearly with temperature and frequency. Obvious mechanisms leading to nonlinear microwave response like Josephson coupling across grain boundaries, nonlocal or nonequilibrium effects cannot explain the data. The anomalies could rather reflect the specific charge and spin ordering and transport phenomena in the low-dimensional cuprate superconductors.",0105613v1 2002-01-25,The influence of microstructures and crystalline defects on the superconductivity of MgB2,"This work studies the influence of microstructures and crystalline defects on the superconductivity of MgB2, with the objective to improve its flux pinning. A MgB2 sample pellet that was hot isostatic pressed (HIPed) was found to have significantly increased critical current density (Jc) at high fields than its un-HIPed counterpart. The HIPed sample had a Jc of 10000 A/cm2 in 50000 Oe (5 T) at 5K. This was 20 times higher than that of the un-HIPed sample, and the same as the best Jc reported by other research groups. Microstructures observed in scanning and transmission electron microscopy indicate that the HIP process eliminated porosity present in the MgB2 pellet resulting in an improved intergrain connectivity. Such improvement in intergrain connectivity was believed to prevent the steep Jc drop with magnetic field H that occurred in the un-HIPed MgB2 pellet at H > 45000 Oe (4.5 T) and T = 5 K. The HIP process was also found to disperse the MgO that existed at the grain boundaries of the un-HIPed MgB2 pellet and to generate more dislocations in the HIPed the pellets. These dispersed MgO particles and dislocations improved flux pinning also at H<45000 Oe. The HIPing process was also found to lower the resistivity at room temperature.",0201486v2 2004-04-19,Low temperature transport in granular metals,"We investigate transport in a granular metallic system at large tunneling conductance between the grains. We show that at low temperatures, $T\leq g_T\delta $, where $\delta$ is the single mean energy level spacing in a grain, the coherent electron motion at large distances dominates the physics, contrary to the high temperature ($T > g_T \delta $) behavior where conductivity is controlled by the scales of the order of the grain size. The conductivity of one and two dimensional granular metals, in the low temperature regime, decays with decreasing temperature in the same manner as that in homogeneous disordered metals, indicating thus an insulating behavior. However, even in this temperature regime the granular structure remains important and there is an additional contribution to conductivity coming from short distances. Due to this contribution the metal-insulator transition in three dimensions occurs at the value of tunnel conductance $g_T^C=(1/6\pi)\ln (E_C/\delta)$, where $E_C$ is the charging energy of an isolated grain, and not at the generally expected $g_T^C \propto 1$. Corrections to the density of states of granular metals due to the electron-electron interaction are calculated. Our results compare favorably with the logarithmic dependence of resistivity in the high-$T_c$ cuprate superconductors indicating that these materials may have a granular structure.",0404443v2 2004-10-21,Novel magnetic behavior of single crystalline Er2PdSi3,"We report the results of ac and dc magnetic susceptibility (chi) and electrical resistivity (rho) measurements on the single crystals of Er2PdSi3, crystallizing in an AlB2-derived hexagonal structure, for two orientations H//[0001] and H//[2 -1 -1 0]. For H//[0001], there are apparently two magnetic transitions as revealed by the ac chi data, one close to 7 K attributable to antiferromagnetic ordering and the other around 2 K. However, for H // [2 -1 -1 0], we observe additional features above 7 K (near 11 and 23 K) in the plot of low-field chi(T); also, there is no corresponding anomaly in the rho(T) plot. In this respect, the magnetic behavior of this compound is novel, particularly while compared with other members of this series. The features in ac chi respond differently to the application of a small dc magnetic field for the two directions. As far as low temperature (T= 1.8 and 5 K) isothermal magnetization (M) behaviour is concerned, it exhibits meta-magnetic-like features around 2 kOe saturating at high fields for the former orientation, whereas for the latter, there is no saturation even at 120 kOe. The sign of paramagnetic Curie temperature is different for these two directions. Thus, there is a strong anisotropy in the magnetic behavior. However, interestingly, the rho(T) plots are found to be essentially isotropic, with the data revealing possible formation of magnetic superzone formation below 7 K.",0410532v1 2006-06-22,Metal-insulator transition in Nd$_{1-x}$Eu$_{x}$NiO$_{3}$ compounds,"Polycrystalline Nd$_{1-x}$Eu$_{x}$NiO$_3$ ($0 \leq x \leq 0.5$) compounds were synthesized in order to investigate the character of the metal-insulator (MI) phase transition in this series. Samples were prepared through the sol-gel route and subjected to heat treatments at $\sim$1000 $^\circ$C under oxygen pressures as high as 80 bar. X-ray Diffraction (XRD) and Neutron Powder Diffraction (NPD), electrical resistivity $\rho(T)$, and Magnetization $M(T)$ measurements were performed on these compounds. The results of NPD and XRD indicated that the samples crystallize in an orthorhombic distorted perovskite structure, space group $Pbnm$. The analysis of the structural parameters revealed a sudden and small expansion of $\sim$0.2% of the unit cell volume when electronic localization occurs. This expansion was attributed to a small increase of $\sim$0.003 \AA{} of the average Ni-O distance and a simultaneous decrease of $\sim$$- 0.5^\circ$ of the Ni-O-Ni superexchange angle. The $\rho(T)$ measurements revealed a MI transition occurring at temperatures ranging from $T_{\rm MI}\sim 193$ to 336 K for samples with $x = 0$ and 0.50, respectively. These measurements also show a large thermal hysteresis in NdNiO$_{3}$ during heating and cooling processes suggesting a first-order character of the phase transition at $T_{\rm MI}$. The width of this thermal hysteresis was found to decrease appreciably for the sample Nd$_{0.7}$Eu$_{0.3}$NiO$_{3}$. The results indicate that cation disorder associated with increasing substitution of Nd by Eu is responsible for changing the first order character of the transition in NdNiO$_{3}$.",0606573v1 2007-03-21,Dynamics of the Magnetic Flux Trapped in Fractal Clusters of a Normal Phase in Percolative Superconductors,"The effect of the fractal clusters of a normal phase, which act as pinning centers, on the dynamics of magnetic flux in percolative type-II superconductor is considered. The main features of these clusters are studied in detail: the cluster statistics is analyzed; the fractal dimension of their boundary is estimated; the distribution of critical currents is obtained, and its peculiarities are explored. It is found that there is the range of fractal dimension where this distribution has anomalous statistical properties, specifically, its dispersion becomes infinite. It is examined how the finite resolution capacity of the cluster geometric size measurement affects the estimated value of fractal dimension. The effect of fractal properties of the normal phase clusters on the electric field arisen from magnetic flux motion is investigated for the cluster area distribution of different kinds. The voltage-current characteristics of fractal superconducting structures in the resistive state are obtained for an arbitrary fractal dimension. It is revealed that the fractality of the boundaries of the normal phase clusters intensifies the magnetic flux trapping and thereby raises the critical current of a superconductor.",0703541v1 2007-03-27,Diffusion and activation of n-type dopants in germanium,"The diffusion and activation of $n$-type impurities (P and As) implanted into $p$-type Ge(100) substrates were examined under various dose and annealing conditions. The secondary ion mass spectrometry profiles of chemical concentrations indicated the existence of a sufficiently high number of impurities with increasing implanted doses. However, spreading resistance probe profiles of electrical concentrations showed electrical concentration saturation in spite of increasing doses and indicated poor activation of As relative to P in Ge. The relationships between the chemical and electrical concentrations of P in Ge and Si were calculated, taking into account the effect of incomplete ionization. The results indicated that the activation of P was almost the same in Ge and Si. The activation ratios obtained experimentally were similar to the calculated values, implying insufficient degeneration of Ge. The profiles of P in Ge substrates with and without damage generated by Ge ion implantation were compared, and it was clarified that the damage that may compensate the activated $n$-type dopants has no relationship with the activation of P in Ge.",0703708v3 2008-10-14,Superconductivity in Fluorine-Arsenide Sr_{1-x}La_xFeAsF,"Since the discovery of superconductivity\cite{1} at 26 K in oxy-pnictide $LaFeAsO_{1-x}F_x$, enormous interests have been stimulated in the fields of condensed matter physics and material sciences. Among the five different structures in this broad type of superconductors\cite{2,3,4,5,6}, the ZrCuSiAs structure has received special attention since the $T_c$ has been quickly promoted to 55-56 K\cite{7,8,9,10,11} in fluorine doped oxy-pnictides REFeAsO (RE = rare earth elements). The superconductivity can also be induced by applying a high pressure to the undoped samples\cite{12,13}. The mechanism of superconductivity in the FeAs-based system remains unclear yet, but it turns out to be clear that any change to the structure or the building blocks will lead to a change of the superconducting transition temperatures. In this Letter, we report the fabrication of the new family of compounds, namely fluorine-arsenides DvFeAsF (Dv = divalent metals) with the ZrCuSiAs structure and with the new building block DvF instead of the REO (both the layers DvF and REO have the combined cation state of ""+1""). The undoped parent phase has a Spin-Density-Wave like transition at about 173 K for SrFeAsF, 118 K for CaFeAsF and 153 K for EuFeAsF. By doping electrons into the system the resistivity anomaly associated with this SDW transition is suppressed and superconductivity appears at 32 K in the fluorine-arsenide Sr$_{1-x}$La$_x$FeAsF (x = 0.4). Our discovery here initiates a new method to obtain superconductors in the FeAs-based system.",0810.2531v3 2009-07-09,Annular Spin-Transfer Memory Element,"An annular magnetic memory that uses a spin-polarized current to switch the magnetization direction or helicity of a magnetic region is proposed. The device has magnetic materials in the shape of a ring (1 to 5 nm in thickness, 20 to 250 nm in mean radius and 8 to 100 nm in width), comprising a reference magnetic layer with a fixed magnetic helicity and a free magnetic layer with a changeable magnetic helicity. These are separated by a thin non-magnetic layer. Information is written using a current flowing perpendicular to the layers, inducing a spin-transfer torque that alters the magnetic state of the free layer. The resistance, which depends on the magnetic state of the device, is used to read out the stored information. This device offers several important advantages compared to conventional spin-transfer magnetic random access memory (MRAM) devices. First, the ring geometry offers stable magnetization states, which are, nonetheless, easily altered with short current pulses. Second, the ring geometry naturally solves a major challenge of spin-transfer devices: writing requires relatively high currents and a low impedance circuit, whereas readout demands a larger impedance and magnetoresistance. The annular device accommodates these conflicting requirements by performing reading and writing operations at separate read and write contacts placed at different locations on the ring.",0907.1600v1 2009-09-16,Band structure engineering of epitaxial graphene on SiC by molecular doping,"Epitaxial graphene on SiC(0001) suffers from strong intrinsic n-type doping. We demonstrate that the excess negative charge can be fully compensated by non-covalently functionalizing graphene with the strong electron acceptor tetrafluorotetracyanoquinodimethane (F4-TCNQ). Charge neutrality can be reached in monolayer graphene as shown in electron dispersion spectra from angular resolved photoemission spectroscopy (ARPES). In bilayer graphene the band gap that originates from the SiC/graphene interface dipole increases with increasing F4-TCNQ deposition and, as a consequence of the molecular doping, the Fermi level is shifted into the band gap. The reduction of the charge carrier density upon molecular deposition is quantified using electronic Fermi surfaces and Raman spectroscopy. The structural and electronic characteristics of the graphene/F4-TCNQ charge transfer complex are investigated by X-ray photoelectron spectroscopy (XPS) and ultraviolet photoelectron spectroscopy (UPS). The doping effect on graphene is preserved in air and is temperature resistant up to 200\degree C. Furthermore, graphene non-covalent functionalization with F4-TCNQ can be implemented not only via evaporation in ultra-high vacuum but also by wet chemistry.",0909.2966v2 2010-01-07,"Anisotropic Connectivity and its Influence on Critical Current Densities, Irreversibility Fields, and Flux Creep in In-Situ-Processed MgB2 Strands","The anisotropy of the critical current density (Jc) and its influence on measurement of irreversibility field (Birr) has been investigated for high quality, in-situ MgB2 strands. Comparison of transport and magnetization measurements has revealed the onset of a regime where large differences exist between transport and magnetically measured values of the critical current density and Birr. These effects, initially unexpected due to the lack of crystalline texture in these in-situ processed strands, appear to be due to a fibrous microstructure, connected with the details of the wire fabrication and MgB2 formation reactions. Scanning electron micrographs of in-situ-processed MgB2 monocore strands have revealed a fibrous microstructure. Grains (~100 nm) are randomly oriented, and there is no apparent local texture of the grains. However, this randomly oriented polycrystalline material has a fibrous texture at a larger length scale, with stringers of MgB2 (~ 60 {\mu}m long and ~5 {\mu}m in diameter) partially separated by elongated pores -- the spaces previously occupied by stringers of elemental Mg. This leads to an interpretation of the differences observed in transport and magnetically determined critical currents, in particular a large deviation between the two at higher fields, in terms of different transverse and longitudinal connectivities within the strand. The different values of connectivity also lead to different resistive transition widths, and thus irreversibility field values, as measured by transport and magnetic techniques. Finally, these considerations are seen to influence estimated pinning potentials for the strands.",1001.1030v1 2010-04-21,Determination of the intrinsic ferroelectric polarization in orthorhombic HoMnO3,"Whether large ferroelectric polarization P exists in the orthorhombic HoMnO3 with the E-type antiferromagnetic spin ordering or not remains as one of unresolved, challenging issues in the physics of multiferroics. The issue is closely linked to an intriguing experimental difficulty for determining P of polycrystalline specimens that conventional pyroelectric current measurements performed after a poling procedure under high dc electric fields are subject to large errors due to the problems caused by leakage currents or space charges. To overcome the difficulty, we employed the PUND method, which uses successively the two positive and two negative electrical pulses, to directly measure electrical hysteresis loops in several polycrystalline HoMnO3 specimens below their N\'eel temperatures. We found that all the HoMnO3 samples had similar remnant polarization Pr values at each temperature, regardless of their variations in resistivity, dielectric constant, and pyroelectric current levels. Moreover, Pr of ~0.07 \mu\C/cm2 at 6 K is consistent with the P value obtained from the pyroelectric current measurement performed after a short pulse poling. Our findings suggest that intrinsic P of polycrystalline HoMnO3 can be determined through the PUND method and P at 0 K may reach ~0.24 \mu\C/cm2 in a single crystalline specimen.",1004.3643v1 2010-07-26,Python Regius (Ball Python) shed skin: Biomimetic analogue for function-targeted design of tribo-surfaces,"A major concern in designing tribo-systems is to minimize friction, save energy, and to reduce wear. Satisfying these requirements depends on the integrity of the rubbing surface and its suitability to sliding conditions. As such, designers currently focus on constructing surfaces that are an integral part of the function of the tribo-system. Inspirations for such constructs come from studying natural systems and from implementing natural design rules. One species that may serve as an analogue for design is the Ball python. This is because such a creature while depending on legless locomotion when sliding against various surfaces, many of which are deemed tribologically hostile, doesn't sustain much damage. Resistance to damage in this case originates from surface design features. As such, studying these features and how do they contribute to the control of friction and wear is very attractive for design purposes. In this work we apply a multi scale surface characterization approach to study surface design features of the Python regius that are beneficial to design high quality lubricating surfaces (such as those obtained through plateau honing). To this end, we studied topographical features by SEM and through White Light Interferrometery (WLI). We further probe the roughness of the surface on multi scale and as a function of location within the body. The results are used to draw a comparison to metrological features of commercial cylinder liners obtained by plateau honing.",1007.4419v1 2010-11-09,Phase diagram of iron-arsenide superconductors Ca(Fe1-xCox)2As2 (0 <= x <= 0.2),"Platelet-like single crystals of the Ca(Fe1-xCox)2As2 series having lateral dimensions up to 15 mm and thickness up to 0.5 mm were obtained from the high temperature solution growth technique using Sn flux. Upon Co doping, the c-axis of the tetragonal unit cell decreases, while the a-axis shows a less significant variation. Pristine CaFe2As2 shows a combined spin-density-wave and structural transition near T = 166 K which gradually shifts to lower temperatures and splits with increasing Co-doping. Both transitions terminate abruptly at a critical Co-concentration of xc = 0.075. For x \geq 0.05, superconductivity appears at low temperatures with a maximum transition temperature TC of around 20 K. The superconducting volume fraction increases with Co concentration up to x = 0.09 followed by a gradual decrease with further increase of the doping level. The electronic phase diagram of Ca(Fe1-xCox)2As2 (0 \leq x \leq 0.2) series is constructed from the magnetization and electric resistivity data. We show that the low-temperature superconducting properties of Co-doped CaFe2As2 differ considerably from those of BaFe2As2 reported previously. These differences seem to be related to the extreme pressure sensitivity of CaFe2As2 relative to its Ba counterpart.",1011.2085v1 2011-08-17,Impact of Protostellar Outflow on Star Formation: Effects of Initial Cloud Mass,"Star formation efficiency controlled by the protostellar outflow in a single cloud core is investigated by three-dimensional resistive MHD simulations. Starting from the prestellar cloud core, the star formation process is calculated until the end of the main accretion phase. In the calculations, the mass of the prestellar cloud is parameterized. During the star formation, the protostellar outflow is driven by the circumstellar disk. The outflow extends also in the transverse direction until its width becomes comparable to the initial cloud scale, and thus, the outflow has a wide opening angle of >40 degrees. As a result, the protostellar outflow sweeps up a large fraction of the infalling material and ejects it into the interstellar space. The outflow can eject at most over half of the host cloud mass, significantly decreasing star formation efficiency. The outflow power is stronger in clouds with a greater initial mass. Thus, the protostellar outflow effectively suppresses star formation efficiency in a massive cloud. The outflow weakens significantly and disappears in several free-fall timescales of the initial cloud after the cloud begins to collapse. The natal prestellar core influences the lifetime and size of the outflow. At the end of the main accretion phase, a massive circumstellar disk comparable in mass to the protostar remains. Calculations show that typically, ~30% of the initial cloud mass is converted into the protostar and ~20% remains in the circumstellar disk, while ~40% is ejected into the interstellar space by the protostellar outflow. Therefore, a single cloud core typically has a star formation efficiency of 30-50%.",1108.3564v1 2012-05-02,Negative thermal expansion and antiferromagnetism in the actinide oxypnictide NpFeAsO,"A neptunium analogue of the LaFeAsO tetragonal layered compound has been synthesized and characterized by a variety of experimental techniques. The occurrence of long-range magnetic order below a critical temperature T_N = 57 K is suggested by anomalies in the temperature-dependent magnetic susceptibility, electrical resistivity, Hall coefficient, and specific heat curves. Below T_N, powder neutron diffraction measurements reveal an antiferromagnetic structure of the Np sublattice, with an ordered magnetic moment of 1.70(0.07) \mu_B aligned along the crystallographic c-axis. No magnetic order has been observed on the Fe sublattice, setting an upper limit of about 0.3 \mu_B for the ordered magnetic moment on the iron. High resolution x-ray powder diffraction measurements exclude the occurrence of lattice transformations down to 5 K, in sharp contrast to the observation of a tetragonal-to-orthorhombic distortion in the rare-earth analogues, which has been associated with the stabilization of a spin density wave on the iron sublattice. Instead, a significant expansion of the NpFeAsO lattice parameters is observed with decreasing temperature below T_N, corresponding to a relative volume change of about 0.2% and to an invar behavior between 5 and 20 K. First-principle electronic structure calculations based on the local-spin density plus Coulomb interaction and the local density plus Hubbard-I approximations provide results in good agreement with the experimental findings.",1205.0438v1 2012-09-13,Magnetic phase transitions in single crystals of the chiral helimagnet Cr1/3NbS2,"The chiral helimagnet Cr1/3NbS2 has been investigated by magnetic, transport and thermal properties measurements on single crystals and by first principles electronic structure calculations. From the measured field and temperature dependence of the magnetization for fields applied perpendicular to the c axis, the magnetic phase diagram has been constructed in the vicinity of the phase transitions. A transition from a paramagnetic to a magnetically ordered phase occurs near 120 K. With increasing magnetic field and at temperatures below 120 K, this material undergoes transitions from a helimagnetic to a soliton-lattice phase near 900 Oe, and then to a ferromagnetic phase near 1300 Oe. The transitions are found to strongly affect the electrical transport. The resistivity decreases sharply upon cooling near 120 K, and the spin reorientation from the helimagnetic ground state to the commensurate ferromagnetic state is evident in the magnetoresistance. At high fields a large magnetoresistance (55 % at 140 kOe) is observed near the magnetic transition temperature. Heat capacity and electronic structure calculations show the density of states at the Fermi level is low in the magnetically ordered state. Effects of spin fluctuations are likely important in understanding the behavior of Cr1/3NbS2 near and above the magnetic ordering transitions.",1209.2783v1 2013-04-15,Non-Fermi liquids and the Wiedemann-Franz law,"A general discussion of the ratio of thermal and electrical conductivities in non-Fermi liquid metals is given. In metals with sharp Drude peaks, the relevant physics is correctly organized around the slow relaxation of almost-conserved momenta. While in Fermi liquids both currents and momenta relax slowly, due to the weakness of interactions among low energy excitations, in strongly interacting non-Fermi liquids typically only momenta relax slowly. It follows that the conductivities of such non-Fermi liquids are obtained within a fundamentally different kinematics to Fermi liquids. Among these strongly interacting non-Fermi liquids we distinguish cases with only one almost-conserved momentum, which we term hydrodynamic metals, and with many patchwise almost-conserved momenta. For all these cases, we obtain universal expressions for the ratio of conductivities that violate the Wiedemann-Franz law. We further discuss the case in which long-lived `cold' quasiparticles, in general with unconventional scattering rates, coexist with strongly interacting hot spots, lines or bands. For these cases, we characterize circumstances under which non-Fermi liquid transport, in particular a linear in temperature resistivity, is and is not compatible with the Wiedemann-Franz law. We suggest the likely outcome of future transport experiments on CeCoIn5, YbRh2Si2 and Sr3Ru2O7 at their critical magnetic fields.",1304.4249v3 2014-05-15,Anomalous frequency and temperature dependent scattering and Hund's coupling in the almost quantum critical heavy fermion system CeFe$_2$Ge$_2$,"We present THz range optical conductivity data of a thin film of the near quantum critical heavy fermion compound CeFe$_2$Ge$_2$. Our complex conductivity measurements find a deviation from conventional Drude-like transport in a temperature range previously reported to exhibit unconventional behavior. We calculate the frequency dependent effective mass and scattering rate using an extended Drude model analysis. We find the inelastic scattering rate can be described by a temperature dependent power-law $\omega^{n(T)}$ where $n(T)$ approaches $\sim1.0 \pm 0.2$ at 1.5 K. This is compared to the $\rho \sim T^{1.5}$ behavior claimed in dc resistivity data and the $\rho \sim T^{2}$ expected from Fermi-liquid theory. In addition to a low temperature mass renormalization, we find an anomalous mass renormalization that persists to high temperature. We attribute this to a Hund's coupling in the Fe states in a manner similar to that recently proposed in the ferro-pnictides. CeFe$_2$Ge$_2$ appears to be a very interesting system where one may study the interplay between the usual $4f$ lattice Kondo effect and this Hund's enhanced Kondo effect in the $3d$ states.",1405.4007v3 2014-05-23,Growth and characterization of heteroepitaxial La-substituted BaSnO$_3$ films on SrTiO$_3$ (001) and SmScO$_3$ (110) substrates,"Heteroepitaxial growth of BaSnO$_3$ (BSO) and Ba$_{1-x}$La$_x$SnO$_3$ (x = 7 %) (LBSO) thin films on different perovskite single crystal (SrTiO$_3$ (001) and SmScO$_3$ (110)) substrates has been achieved by Pulsed Laser Deposition (PLD) under optimized deposition conditions. X-ray diffraction measurements indicate that the films on either of these substrates are relaxed due to the large mismatch and present a high degree of crystallinity with narrow rocking curves and smooth surface morphology while analytical quantification by proton induced x-ray emission (PIXE) confirms the stoichiometric La transfer from a polyphasic target, producing films with La contents above the bulk solubility limit. The films show degenerate semiconducting behavior on both substrates, with the observed room temperature resistivities, Hall mobilities and carrier concentrations of 4.4 $m \Omega cm$, 10.11 $cm^2 V^{-1} s^{-1}$, and 1.38 $\cdot 10^{20} cm^{-3}$ on SmScO$_3$ and 7.8 $m \Omega cm$, 5.8 $cm^2 V^{-1} s^{-1}$, and 1.36 $\cdot 10^{20} cm^{-3}$ on SrTiO$_3$ ruling out any extrinsic contribution from the substrate. The superior electrical properties observed on the SmScO3 substrate are attributed to reduction in dislocation density from the lower lattice mismatch.",1405.6233v1 2014-05-31,Scale-Invariant Dissipationless Chiral Transport in Magnetic Topological Insulators beyond the Two-Dimensional Limit,"We investigate the quantum anomalous Hall Effect (QAHE) and related chiral transport in the millimeter-size (Cr0.12Bi0.26Sb0.62)2Te3 films. With high sample quality and robust magnetism at low temperatures, the quantized Hall conductance of e2/h is found to persist even when the film thickness is beyond the two-dimensional (2D) hybridization limit. Meanwhile, the Chern insulator-featured chiral edge conduction is manifested by the non-local transport measurements. In contrast to the 2D hybridized thin film, an additional weakly field-dependent longitudinal resistance is observed in the 10 quintuple-layer film, suggesting the influence of the film thickness on the dissipative edge channel in the QAHE regime. The extension of QAHE into the three-dimensional thickness region addresses the universality of this quantum transport phenomenon and motivates the exploration of new QAHE phases with tunable Chern numbers. In addition, the observation of the scale-invariant dissipationless chiral propagation on a macroscopic scale makes a major stride towards ideal low-power interconnect applications.",1406.0106v2 2014-09-11,High performance solar cells based on graphene-GaAs heterostructures,"The honeycomb connection of carbon atoms by covalent bonds in a macroscopic two-dimensional scale leads to fascinating graphene and solar cell based on graphene/silicon Schottky diode has been widely studied. For solar cell applications, GaAs is superior to silicon as it has a direct band gap of 1.42 eV and its electron mobility is six times of that of silicon. However, graphene/GaAs solar cell has been rarely explored. Herein, we report graphene/GaAs solar cells with conversion efficiency (Eta) of 10.4% and 15.5% without and with anti-reflection layer on graphene, respectively. The Eta of 15.5% is higher than the state of art efficiency for graphene/Si system (14.5%). Furthermore, our calculation points out Eta of 25.8% can be reached by reasonably optimizing the open circuit voltage, junction ideality factor, resistance of graphene and metal/graphene contact. This research strongly support graphene/GaAs hetero-structure solar cell have great potential for practical applications.",1409.3500v3 2014-10-13,Breakdown of Three-dimensional Dirac Semimetal State in pressurized Cd3As2,"We report the first observation of a pressure-induced breakdown of the 3D-DSM state in Cd3As2, evidenced by a series of in-situ high-pressure synchrotron X-ray diffraction (XRD) and single crystal transport measurements. We find that Cd3As2 undergoes a structural phase transition from a metallic tetragonal (T) phase in space group I41/acd to a semiconducting monoclinic (M) phase in space group P21/c at critical pressure 2.57 GPa, above this pressure, an activation energy gap appears, accompanied by distinct switches in Hall resistivity slope and electron mobility. These changes of crystal symmetry and corresponding transport properties manifest the breakdown of the 3D-DSM state in pressurized Cd3As2.",1410.3213v4 2014-11-13,Analysis of viscoelastic soft dielectric elastomer generators operating in an electrical circuit,"A predicting model for soft Dielectric Elastomer Generators (DEGs) must consider a realistic model of the electromechanical behaviour of the elastomer filling, the variable capacitor and of the electrical circuit connecting all elements of the device. In this paper such an objective is achieved by proposing a complete framework for reliable simulations of soft energy harvesters. In particular, a simple electrical circuit is realised by connecting the capacitor, stretched periodically by a source of mechanical work, in parallel with a battery through a diode and with an electrical load consuming the energy produced. The electrical model comprises resistances simulating the effect of the electrodes and of the conductivity current invariably present through the dielectric film. As these devices undergo a high number of electro-mechanical loading cycles at large deformation, the time-dependent response of the material must be taken into account as it strongly affects the generator outcome. To this end, the viscoelastic behaviour of the polymer and the possible change of permittivity with strains are analysed carefully by means of a proposed coupled electro-viscoelastic constitutive model, calibrated on experimental data available in the literature for an incompressible polyacrilate elastomer (3M VHB4910). Numerical results showing the importance of time-dependent behaviour on the evaluation of performance of DEGs for different loading conditions, namely equi-biaxial and uniaxial, are reported in the final section.",1411.3613v2 2014-11-28,Growth control of the oxidation state in vanadium oxide thin films,"Precise control of the chemical valence or oxidation state of vanadium in vanadium oxide thin films is highly desirable for not only fundamental research, but also technological applications that utilize the subtle change in the physical properties originating from the metal- insulator transition (MIT) near room temperature. However, due to the multivalent nature of vanadium and the lack of a good understanding on growth control of the oxidation state, stabilization of phase pure vanadium oxides with a single oxidation state is extremely challenging. Here, we systematically varied the growth conditions to clearly map out the growth window for preparing phase pure epitaxial vanadium oxides by pulsed laser deposition for providing a guideline to grow high quality thin films with well-defined oxidation states of V2(+3)O3, V(+4)O2, and V2(+5)O5. A well pronounced MIT was only observed in VO2 films grown in a very narrow range of oxygen partial pressure P(O2). The films grown either in lower (< 10 mTorr) or higher P(O2) (> 25 mTorr) result in V2O3 and V2O5 phases, respectively, thereby suppressing the MIT for both cases. We have also found that the resistivity ratio before and after the MIT of VO2 thin films can be further enhanced by one order of magnitude when the films are further oxidized by post-annealing at a well-controlled oxidizing ambient. This result indicates that stabilizing vanadium into a single valence state has to compromise with insufficient oxidation of an as grown thin film and, thereby, a subsequent oxidation is required for an improved MIT behavior.",1411.7922v1 2014-12-05,Effects of Oxygen Adsorption on the Surface State of Epitaxial Silicene on Ag(111),"Epitaxial silicene, which is one single layer of silicon atoms packed in a honeycomb structure, demonstrates a strong interaction with the substrate that dramatically affects its electronic structure. The role of electronic coupling in the chemical reactivity between the silicene and the substrate is still unclear so far, which is of great importance for functionalization of silicene layers. Here, we report the reconstructions and hybridized electronic structures of epitaxial 4x4 silicene on Ag(111), which are revealed by scanning tunneling microscopy and angle-resolved photoemission spectroscopy. The hybridization between Si and Ag results in a metallic surface state, which can gradually decay due to oxygen adsorption. X-ray photoemission spectroscopy confirms the decoupling of Si-Ag bonds after oxygen treatment as well as the relatively oxygen resistance of Ag(111) surface, in contrast to 4x4 silicene [with respect to Ag(111)]. First-principles calculations have confirmed the evolution of the electronic structure of silicene during oxidation. It has been verified experimentally and theoretically that the high chemical activity of 4x4 silicene is attributable to the Si pz state, while the Ag(111) substrate exhibits relatively inert chemical behavior.",1412.1887v1 2015-02-10,Ultrafast dynamic conductivity and scattering rate saturation of photoexcited charge carriers in silicon investigated with a midinfrared continuum probe,"We employ ultra-broadband terahertz-midinfrared probe pulses to characterize the optical response of photoinduced charge-carrier plasmas in high-resistivity silicon in a reflection geometry, over a wide range of excitation densities (10^{15}-10^{19} cm^{-3}) at room temperature. In contrast to conventional terahertz spectroscopy studies, this enables one to directly cover the frequency range encompassing the resultant plasma frequencies. The intensity reflection spectra of the thermalized plasma, measured using sum-frequency (up-conversion) detection of the probe pulses, can be modeled well by a standard Drude model with a density-dependent momentum scattering time of approx. 200 fs at low densities, reaching approx. 20 fs for densities of approx. 10^{19} cm^{-3}, where the increase of the scattering rate saturates. This behavior can be reproduced well with theoretical results based on the generalized Drude approach for the electron-hole scattering rate, where the saturation occurs due to phase-space restrictions as the plasma becomes degenerate. We also study the initial sub-picosecond temporal development of the Drude response, and discuss the observed rise in the scattering time in terms of initial charge-carrier relaxation, as well as the optical response of the photoexcited sample as predicted by finite-difference time-domain simulations.",1502.02829v1 2015-03-03,Construction of force measuring optical tweezers instrumentation and investigations of biophysical properties of bacterial adhesion organelles,"Optical tweezers are a technique in which microscopic-sized particles, including living cells and bacteria, can be non-intrusively trapped with high accuracy solely using focused light. The technique has therefore become a powerful tool in the field of biophysics. Optical tweezers thereby provide outstanding manipulation possibilities of cells as well as semi-transparent materials, both non-invasively and non-destructively, in biological systems. In addition, optical tweezers can measure minute forces (< 10-12 N), probe molecular interactions and their energy landscapes, and apply both static and dynamic forces in biological systems in a controlled manner. The assessment of intermolecular forces with force measuring optical tweezers, and thereby the biomechanical structure of biological objects, has therefore considerably facilitated our understanding of interactions and structures of biological systems. Adhesive bacterial organelles, so called pili, mediate adhesion to host cells and are therefore crucial for the initial bacterial-cell contact. Thus, they serve as an important virulence factor. The investigation of pili, both their biogenesis and their expected in vivo properties, brings information that can be of importance for the design of new drugs to prevent bacterial infections, which is crucial in the era of increased bacterial resistance towards antibiotics. In this thesis, an experimental setup of a force measuring optical tweezers system and the results of a number of biomechanical investigations of adhesive bacterial organelles are presented. Force measuring optical tweezers have been used to characterize three different types of adhesive organelles under various conditions, P, type 1, and S pili, which all are expressed by uropathogenic Escherichia coli. A quantitative biophysical force-extension model, built upon the structure and force response, has been developed.",1503.00881v1 2015-03-30,Microbranching in mode-I fracture using large scale simulations of amorphous and perturbed lattice models,"We study the high-velocity regime mode-I fracture instability when small microbranches start to appear near the main crack, using large scale simulations. Some of the features of those microbranches have been reproduced qualitatively in smaller scale studies (using ${\cal O}(10^4)$ atoms) on both a model of an amorphous materials (via the continuous random network model) and using perturbed lattice models. In this study, larger scale simulations (${\cal O}(10^6)$ atoms) were performed using multi-threading computing on a GPU device, in order to achieve more physically realistic results. First, we find that the microbranching pattern appears to be converging with the lattice width. Second, the simulations reproduce the growth of the size of a microbranch as a function of the crack velocity, as well as the increase of the amplitude of the derivative of the electrical resistance RMS with respect to the time as a function of the crack velocity. In addition, the simulations yield the correct branching angle of the microbranches, and the power law governing the shape of the microbranches seems to be lower than one, so that the side cracks turn over in the direction of propagation of the main crack as seen in experiment.",1503.08616v2 2016-04-12,An invisible non-volatile solid-state memory,"Information technologies require entangling data stability with encryption for a next generation of secure data storage. Current magnetic memories, ranging from low-density stripes up to high-density hard drives, can ultimately be detected using routinely available probes or manipulated by external magnetic perturbations. Antiferromagnetic resistors feature unrivalled robustness but the stable resistive states reported scarcely differ by more than a fraction of a percent at room temperature. Here we show that the metamagnetic (ferromagnetic to antiferromagnetic) transition in intermetallic Fe0.50Rh0.50 can be electrically controlled in a magnetoelectric heterostructure to reveal or cloak a given ferromagnetic state. From an aligned ferromagnetic phase, magnetic states are frozen into the antiferromagnetic phase by the application of an electric field, thus eliminating the stray field and likewise making it insensitive to external magnetic field. Application of a reverse electric field reverts the antiferromagnetic state to the original ferromagnetic state. Our work demonstrates the building blocks of a feasible, extremely stable, non-volatile, electrically addressable, low-energy dissipation, magnetoelectric multiferroic memory.",1604.03383v2 2016-05-19,Robust two-dimensional superconductivity and vortex system in Bi2Te3/FeTe heterostructures,"The discovery of two-dimensional superconductivity in Bi2Te3/FeTe heterostructure provides a new platform for the search of Majorana fermions in condensed matter systems. Since Majorana fermions are expected to reside at the core of the vortices, a close examination of the vortex dynamics in superconducting interface is of paramount importance. Here, we report the robustness of the interfacial superconductivity and 2D vortex dynamics in four as-grown and aged Bi2Te3/FeTe heterostructure with different Bi2Te3 epilayer thickness (3, 5, 7, 14 nm). After two years' air exposure, superconductivity remains robust even when the thickness of Bi2Te3 epilayer is down to 3 nm. Meanwhile, a new feature at ~13 K is induced in the aged samples, and the high field studies reveal its relevance to superconductivity. The resistance of all as-grown and aged heterostructures, just below the superconducting transition temperature follows the Arrhenius relation, indicating the thermally activated flux flow behavior at the interface of Bi2Te3 and FeTe. Moreover, the activation energy exhibits a logarithmic dependence on the magnetic field, providing a compelling evidence for the 2D vortex dynamics in this novel system. The weak disorder associated with aging-induced Te vacancies is possibly responsible for these observed phenomena.",1605.05903v1 2016-07-06,Chiral anomaly from strain-induced gauge fields in Dirac and Weyl semimetals,"Dirac and Weyl semimetals form an ideal platform for testing ideas developed in high energy physics to describe massless relativistic particles. One such quintessentially field-theoretic idea of chiral anomaly already resulted in the prediction and subsequent observation of the pronounced negative magnetoresistance in these novel materials for parallel electric and magnetic fields. Here we predict that the chiral anomaly occurs - and has experimentally observable consequences - when real electromagnetic fields E and B are replaced by strain-induced pseudo-electromagnetic fields e and b. For example, a uniform pseudomagnetic field b is generated when a Weyl semimetal nanowire is put under torsion. In accord with the chiral anomaly equation we predict a negative contribution to the wire resistance proportional to the square of the torsion strength. Remarkably, left and right moving chiral modes are then spatially segregated to the bulk and surface of the wire forming a ""topological coaxial cable"". This produces hydrodynamic flow with potentially very long relaxation time. Another effect we predict is the ultrasonic attenuation and electromagnetic emission due to a time periodic mechanical deformation causing pseudoelectric field e. These novel manifestations of the chiral anomaly are most striking in the semimetals with a single pair of Weyl nodes but also occur in Dirac semimetals such as Cd3As2 and Na3Bi and Weyl semimetals with unbroken time reversal symmetry.",1607.01810v2 2016-11-17,Interfacial thermal conductance in graphene/black phosphorus heterogeneous structures,"Graphene, as a passivation layer, can be used to protect the black phosphorus from the chemical reaction with surrounding oxygen and water. However, black phosphorus and graphene heterostructures have low efficiency of heat dissipation due to its intrinsic high thermal resistance at the interfaces. The accumulated energy from Joule heat has to be removed efficiently to avoid the malfunction of the devices. Therefore, it is of significance to investigate the interfacial thermal dissipation properties and manipulate the properties by interfacial engineering on demand. In this work, the interfacial thermal conductance between few-layer black phosphorus and graphene is studied extensively using molecular dynamics simulations. Two critical parameters, the critical power Pcr to maintain thermal stability and the maximum heat power density Pmax with which the system can be loaded, are identified. Our results show that interfacial thermal conductance can be effectively tuned in a wide range with external strains and interracial defects. The compressive strain can enhance the interfacial thermal conductance by one order of magnitude, while interface defects give a two-fold increase. These findings could provide guidelines in heat dissipation and interfacial engineering for thermal conductance manipulation of black phosphorus-graphene heterostructure-based devices.",1611.05598v1 2017-06-08,Electronic and phonon excitations in α-RuCl$_3$,"We report on THz, infrared reflectivity and transmission experiments for wave numbers from 10 to 8000 cm$^{-1}$ ($\sim$ 1 meV - 1 eV) and for temperatures from 5 to 295 K on the Kitaev candidate material {\alpha}-RuCl$_3$. As reported earlier, the compound under investigation passes through a first-order structural phase transition, from a monoclinic high-temperature to a rhombohedral low-temperature phase. The phase transition shows an extreme and unusual hysteretic behavior, which extends from 60 to 166 K. In passing this phase transition, in the complete frequency range investigated we found a significant reflectance change, which amounts almost a factor of two. We provide a broadband spectrum of dielectric constant, dielectric loss and optical conductivity from the THz to the mid infrared regime and study in detail the phonon response and the low-lying electronic density of states. We provide evidence for the onset of an optical energy gap, which is of order 200 meV, in good agreement with the gap derived from measurements of the DC electrical resistivity. Remarkably, the onset of the gap exhibits a strong blue shift on increasing temperatures.",1706.02724v2 2017-10-03,Holographic model for the anomalous scalings of the cuprates,"We examine transport in a holographic model in which the dynamics of the charged degrees of freedom is described by the nonlinear Dirac-Born-Infeld (DBI) action. Axionic scalar fields are included to break translational invariance and generate momentum dissipation in the system. Scaling exponents are introduced by using geometries which are nonrelativistic and hyperscaling-violating in the infrared. In the probe DBI limit the theory reproduces the anomalous temperature dependence of the resistivity and Hall angle of the cuprate strange metals, $\rho \sim T$ and $\cot\Theta_H \sim T^2$. These scaling laws would not be present without the nonlinear dynamics encoded by the DBI interactions. We further show that because of its richness the DBI theory supports a wide spectrum of temperature scalings. This model provides explicit examples in which transport is controlled by different relaxation times. On the other hand, when only one quantity sets the temperature scale of the system, the Hall angle and conductivity typically exhibit the same temperature behavior. We illustrate this point using new fully backreacted analytical dyonic black brane solutions.",1710.01326v2 2018-01-31,The origin of Mooij correlations in disordered metals,"Sufficiently disordered metals display systematic deviations from the behavior predicted by semi-classical Boltzmann transport theory. Here the scattering events from impurities or thermal excitations can no longer be considered as additive independent processes, as asserted by Matthiessen's rule following from this picture. In the intermediate region between the regime of good conduction and that of insulation, one typically finds a change of sign of the temperature coefficient of resistivity (TCR), even at elevated temperature spanning ambient conditions, a phenomenology that was first identified by Mooij in 1973. Traditional weak coupling approaches to identify relevant corrections to the Boltzmann picture focused on long distance interference effects such as ""weak localization"", which are especially important in low dimensions (1D, 2D) and close to the zero temperature limit. Here we formulate a strong-coupling approach to tackle the interplay of strong disorder and lattice deformations (phonons) in bulk three-dimensional metals at high temperatures. We identify a polaronic mechanism of strong disorder renormalization, which describes how a lattice locally responds to the relevant impurity potential. This mechanism, which quantitatively captures the Mooij regime, is physically distinct and unrelated to Anderson localization, but realizes early seminal ideas of Anderson himself, concerning the interplay of disorder and lattice deformations.",1802.00065v4 2018-05-30,Hikami-Larkin-Nagaoka (HLN) treatment of the Magneto Conductivity of Bi2Te3 Topological Insulator,"We report the magneto-conductivity analysis at different temperatures under magnetic field of up to 5Tesla of a well characterized Bi2Te3 crystal. Details of crystal growth and various physical properties including high linear magneto resistance are already reported by some of us. To elaborate upon the transport properties of Bi2Te3 crystal, the magneto conductivity is fitted to the known HLN (Hikami Larkin Nagaoka) equation and it is found that the conduction mechanism is dominated by both surface driven WAL (weak anti localization) and the bulk WL states. The value of HLN equation coefficient signifying the type of localization (WL, WAL or both WL and WAL) falls within the range of -0.5 to -1.5. In our case, the low field (0.25Tesla) fitting of studied crystal exhibited value close to -0.86 for studied temperatures of up to 50K, indicating both WAL and WL contributions. The phase coherence length is found to decrease from 98.266 to 40.314nm with increasing temperature. Summarily, the short letter reports the fact that bulk Bi2Te3 follows the HLN equation and quantitative analysis of the same facilitates to know the quality of studied crystal in terms of WAL to WL contributions and thus the surface to bulk conduction ratio.",1805.11822v1 2018-06-18,Band structure and Fermi surfaces of the reentrant ferromagnetic superconductor Eu(Fe0.86Ir0.14)2As2,"The electronic structure of the reentrant superconductor Eu(Fe$_{0.86}$Ir$_{0.14}$)$_{2}$As$_{2}$ (T$_c$ = 22 K) with coexisting ferromagnetic order (T$_M$ = 18 K) is investigated using angle-resolved photoemission spectroscopy (ARPES) and scanning tunneling spectroscopy (STS). We study the in-plane and out-of-plane band dispersions and Fermi surface (FS) of Eu(Fe$_{0.86}$Ir$_{0.14}$)$_{2}$As$_{2}$. The near E$_F$ Fe 3d-derived band dispersions near the $\Gamma$ and X high-symmetry points show changes due to Ir substitution, but the FS topology is preserved. From momentum dependent measurements of the superconducting gap measured at T = 5 K, we estimate an essentially isotropic s-wave gap ($\Delta\sim5.25\pm 0.25$ meV), indicative of strong-coupling superconductivity with 2$\Delta$/k$_{B}$T$_{c}\simeq$ 5.8. The gap gets closed at temperatures T $\geq$ 10 K, and this is attributed to the resistive phase which sets in at T$_M$ = 18 K due to the Eu$^{2+}$-derived magnetic order. The modifications of the FS with Ir substitution clearly indicates an effective hole doping with respect to the parent compound.",1806.06563v1 2018-09-26,Nanoscale Intergranular Corrosion and Relation With Grain Boundary Character as Studied In Situ on Copper,"The initiation of intergranular corrosion at various types of grain boundaries (GBs) was studied at the nanometer scale on microcrystalline copper in 1 mM HCl aqueous solution. In situ Electrochemical Scanning Tunneling Microscopy (ECSTM) and Electron Back-Scatter Diffraction analysis of the same local microstructural region were combined using an innovative methodology including micro marking performed with the STM tip. The results demonstrate that electrochemically-induced intergranular dissolution, at the surface termination of GBs, is dependent on the grain boundary character. It is found that random high angle boundaries as well as sigma9 coincidence site lattice (CSL) boundaries are susceptible to nanoscale initiation of intergranular corrosion while for sigma3 CSL boundaries the behavior is dependent on the deviation angle of the GB plane from the exact orientation. For the sigma3 twins, a transition from resistance to susceptibility occurs between 1{\deg} and 1.7{\deg} of deviation as a result of the increase of the density of steps (i.e. misorientation dislocations) in the coincidence boundary plane. The work emphasizes the precision needed in the design of the grain boundary network in applications where intergranular corrosion or its initiation must be controlled at the nanoscale.",1809.09872v1 2018-11-14,Multifrequency Nanoscale Impedance Microscopy (m-NIM): A novel approach towards detection of selective and subtle modifications on the surface of polycrystalline boron-doped diamond electrodes,"In this paper, we describe the modification of Nanoscale Impedance Microscopy (NIM), namely, a combination of contact-mode atomic force microscopy with local impedance measurements. The postulated approach is based on the application of multifrequency voltage perturbation instead of standard frequency-by-frequency analysis, which among others offers more time-efficient and accurate determination of the resultant impedance spectra with high spatial resolution. Based on the impedance spectra analysis with an appropriate electric equivalent circuit, it was possible to map surface resistance and contact capacitance. Polycrystalline heavy boron-doped diamond (BDD) electrodes were the research object. Recent studies have shown that the exposure of such electrodes to oxidizing environment may result in the modification of termination type, and thus it is a key factor in describing the electric and electrochemical properties of BDD. We have successfully applied multifrequency NIM, which allowed us to prove that the modification of termination type is selective and occurs with different propensity on the grains having specific crystallographic orientation. Furthermore, our approach enabled the detection of even subtle submicroscopic surface heterogeneities, created as a result of various oxidation treatments and to distinguish them from the surface heterogeneity related to the local distribution of boron at the grain boundaries.",1811.05709v1 2019-05-12,Nodeless superconductivity and preserved time-reversal symmetry in the noncentrosymmetric Mo3P superconductor,"We report a comprehensive study of the noncentrosymmetric superconductor Mo$_3$P. Its bulk superconductivity, with $T_c = 5.5$ K, was characterized via electrical resistivity, magnetization, and heat-capacity measurements, while its microscopic electronic properties were investigated by means of muon-spin rotation/relaxation ($\mu$SR) and nuclear magnetic resonance (NMR) techniques. In the normal state, NMR relaxation data indicate an almost ideal metallic behavior, confirmed by band-structure calculations, which suggest a relatively high electron density of states, dominated by the Mo $4d$-orbitals. The low-temperature superfluid density, determined via transverse-field $\mu$SR and electronic specific heat, suggest a fully-gapped superconducting state in Mo$_3$P, with $\Delta_0= 0.83$ meV, the same as the BCS gap value in the weak-coupling case, and a zero-temperature magnetic penetration depth $\lambda_0 = 126$ nm. The absence of spontaneous magnetic fields below the onset of superconductivity, as determined from zero-field $\mu$SR measurements, indicates a preserved time-reversal symmetry in the superconducting state of Mo$_3$P and, hence, spin-singlet pairing.",1905.04726v1 2019-05-28,Electronic structure and $H$-$T$ phase diagram of Eu(Fe$_{1-x}$Rh$_x$)$_2$As$_2$,"The iron-based superconductors represent a promising platform for high-temperature superconductivity, but the interactions underpinning their pairing present a puzzle. The EuFe$_2$As$_2$ family is unique among these materials for having magnetic order which onsets within the superconducting state, just below the superconducting transition. Superconductivity and magnetic order are normally antagonistic and often vie for the same unpaired electrons, but in this family the magnetism arises from largely localized Eu moments and they coexist, with the competition between these evenly-matched opponents leading to reentrant superconducting behavior. To help elucidate the physics in this family and the interactions between the magnetic order and superconductivity, we investigate the $H$--$T$ phase diagram near optimal Rh doping through specific heat, resistivity, and magnetization measurements, and study the electronic structure by angular-resolved photoemission spectroscopy. The competition between the Eu and FeAs layers may offer a route to directly accessing the electronic structure under effective magnetic fields via ARPES, which is ordinarily a strictly zero-field technique.",1905.11554v2 2019-09-10,New and fast route to black TiO2 based on hollow cathode H2 plasma,"In this work, we demonstrate a new method to produce black TiO2 from pristine anatase TiO2 films. It consists on the immersion of TiO2 films in a hollow cathode H2 RF plasma for a few minutes, resulting in an efficient blackening of TiO2. In this study, the pristine anatase TiO2 films were grown by magnetron sputtering onto cover glass and c-Si substrates and then annealed at 450 {\deg}C for 2 h. Before and after the hollow cathode H2 plasma treatment, the samples were characterized by profilometry, UV-Vis spectrophotometry, X-ray diffraction, Raman spectroscopy, X-ray photoelectron spectroscopy, field emission scanning electron and atomic force microscopies, and four-point probe measurements. The results show that the obtained black TiO2 thin films have a significant light absorption on the whole solar spectrum, a very low sheet resistance, and also a relatively high surface area when compared to the pristine TiO2. All these characteristics lead to an important improvement on their photocatalytic activity, as measured by the degradation rate of methylene blue under UV irradiation.",1909.04623v1 2019-09-27,Superconducting proximity effect in InAsSb surface quantum wells with in-situ Al contact,"We demonstrate robust superconducting proximity effect in InAs$_{0.5}$Sb$_{0.5}$ quantum wells grown with epitaxial Al contact, which has important implications for mesoscopic and topological superconductivity. Unlike more commonly studied InAs and InSb semiconductors, bulk InAs$_{0.5}$Sb$_{0.5}$ supports stronger spin-orbit coupling and larger $g$-factor. However, these potentially desirable properties have not been previously measured in epitaxial heterostructures with superconductors, which could serve as a platform for fault-tolerant topological quantum computing. Through structural and transport characterization we observe high-quality interfaces and strong spin-orbit coupling. We fabricate Josephson junctions based on InAs$_{0.5}$Sb$_{0.5}$ quantum wells and observe strong proximity effect. These junctions exhibit product of normal resistance and critical current, $I_{c}R_{N} = \SI{270}{\micro V}$, and excess current, $I_{ex}R_{N} = \SI{200}{\micro V}$ at contact separations of 500~nm. Both of these quantities demonstrate a robust and long-range proximity effect with highly-transparent contacts.",1909.12571v2 2020-03-15,Vacancy diffusion in multi-principal element alloys: the role of chemical disorder in the ordered lattice,"Many of the purported virtues of Multi-Principal Element Alloys (MPEAs), such as corrosion, high-temperature oxidation and irradiation resistance, are highly sensitive to vacancy diffusivity. Similarly, solute interdiffusion is governed by vacancy diffusion -- it is often unclear whether MPEAs are truly stable, or effectively stabilized by slow interdiffusion. The considerable composition space afforded to these alloys makes optimizing for desired properties a daunting task; theoretical and computational tools are necessary to guide alloy development. For diffusion, such tools depend on both a knowledge of the vacancy migration barriers within a given alloy and an understanding of how these barriers influence vacancy diffusivity. We present a generalized theory of vacancy diffusion in rugged energy landscapes, paired with Kinetic Monte Carlo simulations of MPEA vacancy diffusion. The barrier energy statistics are informed by nudged elastic band calculations in the equiatomic CoNiCrFeMn alloy. Theory and simulations show that vacancy diffusion in solid-solution MPEAs is not necessarily sluggish, but can potentially be tuned, and that trap models are an insufficient explanation for sluggish diffusion in the CoNiCrFeMn HEA. These results also show that any model that endeavors to faithfully represent diffusion-related phenomena must account for the full nature of the energy landscape, not just the migration barriers.",2003.06900v2 2017-03-28,Indium substitution effect on the topological crystalline insulator family (Pb$_{1-x}$Sn$_{x}$)$_{1-y}$In$_{y}$Te: Topological and superconducting properties,"Topological crystalline insulators (TCIs) have been of great interest in the area of condensed matter physics. We investigated the effect of indium substitution on the crystal structure and transport properties in the TCI system (Pb$_{1-x}$Sn$_{x}$)$_{1-y}$In$_{y}$Te. For samples with a tin concentration $x\le50\%$, the low-temperature resisitivities show a dramatic variation as a function of indium concentration: with up to ~2% indium doping the samples show weak-metallic behavior, similar to their parent compounds; with ~6% indium doping, samples have true bulk-insulating resistivity and present evidence for nontrivial topological surface states; with higher indium doping levels, superconductivity was observed, with a transition temperature, Tc, positively correlated to the indium concentration and reaching as high as 4.7 K. We address this issue from the view of bulk electronic structure modified by the indium-induced impurity level that pins the Fermi level. The current work summarizes the indium substitution effect on (Pb,Sn)Te, and discusses the topological and superconducting aspects, which can be provide guidance for future studies on this and related systems.",1703.09836v1 2019-02-22,Development of transmon qubits solely from optical lithography on 300mm wafers,"Qubit information processors are increasing in footprint but currently rely on e-beam lithography for patterning the required Josephson junctions (JJs). Advanced optical lithography is an alternative patterning method, and we report on the development of transmon qubits patterned solely with optical lithography. The lithography uses 193 nm wavelength exposure and 300-mm large silicon wafers. Qubits and arrays of evaluation JJs were patterned with process control which resulted in narrow feature distributions: a standard deviation of 0:78% for a 220 nm linewidth pattern realized across over half the width of the wafers. Room temperature evaluation found a 2.8-3.6% standard deviation in JJ resistance in completed chips. The qubits used aluminum and titanium nitride films on silicon substrates without substantial silicon etching. T1 times of the qubits were extracted at 26 - 27 microseconds, indicating a low level of material-based qubit defects. This study shows that large wafer optical lithography on silicon is adequate for high-quality transmon qubits, and shows a promising path for improving many-qubit processors.",1902.08501v1 2019-06-30,Evaluating Superconductors through Current Induced Depairing,"The phenomenon of superconductivity occurs in the phase space of three principal parameters: temperature T, magnetic field B, and current density Jd . The critical temperature Tc is one of the first parameters that is measured and in a certain way defines the superconductor. From the practical applications point of view, of equal importance is the upper critical magnetic field Bc2 and conventional critical current density Jc (above which the system begins to show resistance without entering the normal state). However, a seldom-measured parameter, the depairing current density Jd , holds the same fundamental importance as Tc and Bc2, in that it defines a boundary between the superconducting and normal states. A study of Jd sheds unique light on other important characteristics of the superconducting state such as the superfluid density and the nature of the normal state below Tc, information that can play a key role in better understanding newly-discovered superconducting materials. From a measurement perspective, the extremely high values of Jd make it difficult to measure, which is the reason why it is seldom measured. Here, we will review the fundamentals of current-induced depairing and the fast-pulsed current technique that facilitates its measurement and discuss the results of its application to the topological-insulator/chalcogenide interfacial superconducting system. Keywords: pairbreaking, pair-breaking, vortex, vortices, theory, tutorial, RTS, room-temperature supeconductivity",1907.00427v1 2019-07-29,Imaging Nematic Transitions in Iron-Pnictide Superconductors with a Quantum Gas,"The SQCRAMscope is a recently realized Scanning Quantum CRyogenic Atom Microscope that utilizes an atomic Bose-Einstein condensate to measure magnetic fields emanating from solid-state samples. The quantum sensor does so with unprecedented DC sensitivity at micron resolution from room-to-cryogenic temperatures. An additional advantage of the SQCRAMscope is the preservation of optical access to the sample: Magnetometry imaging of, e.g., electron transport may be performed in concert with other imaging techniques. This multimodal imaging capability can be brought to bear with great effect in the study of nematicity in iron-pnictide high-temperature superconductors, where the relationship between electronic and structural symmetry-breaking resulting in a nematic phase is under debate. Here, we combine the SQCRAMscope with an in situ microscope that measures optical birefringence near the surface. This enables simultaneous and spatially resolved detection of both bulk and near-surface manifestations of nematicity via transport and structural deformation channels, respectively. By performing the first local measurement of emergent resistivity anisotropy in iron pnictides, we observe sharp, nearly concurrent transport and structural transitions. More broadly, these measurements demonstrate the SQCRAMscope's ability to reveal important insights into the physics of complex quantum materials.",1907.12601v2 2020-02-05,Impact of Residual Carbon Impurities and Gallium Vacancies on Trapping Effects in AlGaN/GaN MIS-HEMTs,"Effects of residual C impurities and Ga vacancies on the dynamic instabilities of AlN/AlGaN/GaN metal insulator semiconductor high electron mobility transistors are investigated. Secondary ion mass spectroscopy, positron annihilation spectroscopy, steady state and time-resolved photoluminescence (PL) measurements have been performed in conjunction with electrical characterization and current transient analyses. The correlation between yellow luminescence (YL), C- and Ga vacancy concentration is investigated. Time-resolved PL indicating the C$_{\mathrm{N}}$O$_{\mathrm{N}}$ complex as the main source of the YL, while Ga vacancies or related complexes with C seem not to play a major role. The device dynamic performance is found to be significantly dependent on the C concentration close to the channel of the transistor. Additionally, the magnitude of the YL is found to be in agreement with the threshold voltage shift and with the on-resistance degradation. Trap analysis of the GaN buffer shows an apparent activation energy of $\sim$0.8eV for all samples, pointing to a common dominating trapping process and that the growth parameters affect solely the density of trap centres. It is inferred that the trapping process is likely to be directly related to C based defects.",2002.01952v1 2020-04-17,Magnetic correlations in subsystems of the misfit [Ca$_2$CoO$_3$]$_{0.62}$[CoO$_2$] cobaltate,"[Ca$_2$CoO$_3$]$_{0.62}$[CoO$_2$], a two dimensional misfit metallic compound, is famous for its rich phases accessed by temperature, $i.e.$ high temperature spin-state transition, metal-insulator transition (MIT) at intermediate temperature ($\sim$ 100 K) and low temperature spin density wave (SDW). It enters into SDW phase below T$_{MIT}$ which becomes long range at 27 K. Information on the independent role of misfit layers (rocksalt/Ca$_2$CoO$_3$ \& triangular/CoO$_2$) in these phases is scarce. By combining a set of complementary macroscopic (DC magnetization and resistivity) and microscopic (neutron diffraction and X-ray absorption fine structure spectroscopy) measurements on pure (CCO) and Tb substituted in the rocksalt layer of CCO (CCO1), magnetic correlations in both subsystems of this misfit compound are unraveled. CCO is found to exhibit glassiness, as well as exchange bias (EB) effects, while CCO1 does not exhibit glassiness, albeit it shows weaker EB effect. By combining local structure investigations from extended X-ray absorption fine structure (EXAFS) spectroscopy and neutron diffraction results on CCO, we confirm that the SDW arises in the CoO$_2$ layer. Our results show that the magnetocrystalline anisotropy associated with the rocksalt layer acts as a source of pinning, which is responsible for EB effect. Ferromagnetic clusters in the Ca$_2$CoO$_3$ affects SDW in CoO$_2$ and ultimately glassiness arises.",2004.08319v2 2020-08-31,Electronic properties in itinerant ferromagnet SrRu$_{1-x}$Ti$_x$O$_3$,"Here, we study the electrical transport and specific heat in 4$d$ based ferromagnetic material SrRuO$_3$ and its Ti substituted SrRu$_{1-x}$Ti$_x$O$_3$ series ($x$ $\le$ 0.7). The SrRuO$_3$ is a metal and shows itinerant ferromagnetism with transition temperature $T_c$ $\sim$ 160 K. The nonmagnetic Ti$^{4+}$ (3$d^0$) substitution would not only weaken the active Ru-O-Ru channel but is also expected to tune the electronic density and electron correlation effect. A metal to insulator transition has been observed around $x$ $\sim$ 0.4. The nature of charge transport in paramagnetic-metallic state ($x$ $\leq$ 0.4) and in insulating state ($x$ $>$ 0.4) follows modified Mott's variable range hopping model. In ferromagnetic-metallic state, resistivity shows a $T^2$ dependence below $T_c$ which though modifies to $T^{3/2}$ dependence at low temperature. In Ti substituted samples, temperature range for $T^{3/2}$ dependence extends to higher temperature. Interestingly, this $T^{3/2}$ dependence dominates in whole ferromagnetic regime in presence of magnetic field. This evolution of electronic transport behavior can be explained within the framework of Fermi liquid theory and electron-magnon scattering mechanism. The negative magnetoresistance exhibits a hysteresis and a crossover between negative and positive value with magnetic field which is connected with magnetic behavior in series. The decreasing electronic coefficient of specific heat with $x$ supports the increasing insulating behavior in present series. We calculate a high Kadowaki-Woods ratio ($x$ $\leq$ 0.3) for SrRuO$_3$ which increases with substitution concentration. This signifies an increasing electronic correlation effect with substitution concentration.",2009.00076v1 2007-10-21,Change of strength of vortex pinning in YBCO due to BaZrO_3 inclusions,"We probe the short-range pinning properties with the application of microwave currents at very high driving frequencies (47.7 GHz) on YBa$_2$Cu$_3$O$_{7-\delta}$ films with and without sub-micrometer BaZrO$_3$ inclusions. We explore the temperature and field ranges 60 K$MOhm resistance at zero charge density and zero displacement field, where the tight-binding calculation predicts a metallic ground state. By increasing the displacement field, we observed a Chern insulator state with C = -5 and two other states with C = -3 at a low magnetic field of ~1 Tesla. At high displacement fields and charge densities, we observed isospin-polarized quarter- and half-metals. Therefore, rhombohedral-stacked pentalayer graphene is the first graphene system to exhibit two different types of Fermi-surface instabilities: driven by a pair of flat bands touching at zero energy, and by the Stoner mechanism in a single flat band. Our results demonstrate a new direction to explore intertwined electron correlation and topology phenomena in natural graphitic materials without the need of moir\'e superlattice engineering.",2305.03151v2 2023-05-10,Strange metallicity in an antiferromagnetic quantum critical model: A sign-problem-free quantum Monte-Carlo study,"We compute transport and thermodynamic properties of a two-band spin-fermion model describing itinerant fermions in two dimensions interacting via $Z_2$ antiferromagnetic quantum critical fluctuations by means of a sign-problem-free quantum Monte-Carlo approach. We show that the phase diagram of this model indeed contains a $d$-wave superconducting phase at low enough temperatures. However, a crucial question that arises is whether a non-Fermi-liquid metallic regime exists above $T_c$ exhibiting hallmark strange-metal transport phenomenology. Interestingly, we find that this version of the model describes a non-Fermi-liquid metallic regime that displays an approximately $T$-linear resistivity above $T_c$ for a strong fermion-boson interaction. Using Nernst-Einstein relation, our QMC results also show that this strange metal phase exhibits a crossover from being characterized by a charge compressibility given approximately by $\chi_{c}\sim 1/T$ at high temperatures to being described by a charge diffusivity consistent with the scaling $D_{c}\sim 1/T$ at low temperatures. Therefore, our work adds support to the view that the $Z_2$ antiferromagnetic spin-fermion model at strong coupling can be considered a minimal model that describes both unconventional superconductivity and strange metallicity, which are fundamentally interconnected in many important strongly-correlated quantum materials.",2305.06421v2 2023-06-09,Giant Hall Switching by Surface-State-Mediated Spin-Orbit Torque in a Hard Ferromagnetic Topological Insulator,"Topological insulators (TI) and magnetic topological insulators (MTI) can apply highly efficient spin-orbit torque (SOT) and manipulate the magnetization with their unique topological surface states with ultra-high efficiency. Here, we demonstrate efficient SOT switching of a hard MTI, V-doped (Bi,Sb)2Te3 (VBST) with a large coercive field that can prevent the influence of an external magnetic field. A giant switched anomalous Hall resistance of 9.2 $k\Omega$ is realized, among the largest of all SOT systems. The SOT switching current density can be reduced to $2.8\times10^5 A/cm^2$. Moreover, as the Fermi level is moved away from the Dirac point by both gate and composition tuning, VBST exhibits a transition from edge-state-mediated to surface-state-mediated transport, thus enhancing the SOT effective field to $1.56\pm 0.12 T/ (10^6 A/cm^2)$ and the interfacial charge-to-spin conversion efficiency to $3.9\pm 0.3 nm^{-1}$. The findings establish VBST as an extraordinary candidate for energy-efficient magnetic memory devices.",2306.05603v3 2023-06-26,CIMulator: A Comprehensive Simulation Platform for Computing-In-Memory Circuit Macros with Low Bit-Width and Real Memory Materials,"This paper presents a simulation platform, namely CIMulator, for quantifying the efficacy of various synaptic devices in neuromorphic accelerators for different neural network architectures. Nonvolatile memory devices, such as resistive random-access memory, ferroelectric field-effect transistor, and volatile static random-access memory devices, can be selected as synaptic devices. A multilayer perceptron and convolutional neural networks (CNNs), such as LeNet-5, VGG-16, and a custom CNN named C4W-1, are simulated to evaluate the effects of these synaptic devices on the training and inference outcomes. The dataset used in the simulations are MNIST, CIFAR-10, and a white blood cell dataset. By applying batch normalization and appropriate optimizers in the training phase, neuromorphic systems with very low-bit-width or binary weights could achieve high pattern recognition rates that approach software-based CNN accuracy. We also introduce spiking neural networks with RRAM-based synaptic devices for the recognition of MNIST handwritten digits.",2306.14649v1 2023-07-03,Designing impact-resistant bio-inspired low-porosity structures using neural networks,"Biological structural designs in nature, like hoof walls, horns, and antlers, can be used as inspiration for generating structures with excellent mechanical properties. A common theme in these designs is the small percent porosity in the structure ranging from 1 - 5\%. In this work, the sheep horn was used as an inspiration due to its higher toughness when loaded in the radial direction compared to the longitudinal direction. Under dynamic transverse compression, we investigated the structure-property relations in low porosity structures characterized by their two-dimensional (2D) cross-sections. A diverse design space was created by combining polygonal tubules with different numbers of sides placed on a grid with varying numbers of rows and columns. The volume fraction and the orientation angle of the tubules were also varied. The finite element (FE) method was used with a rate-dependent elastoplastic material model to generate the stress-strain curves under plane strain conditions. A gated recurrent unit (GRU) model was trained to predict the structures' stress-strain response and energy absorption under different strain rates and applied strains. The parameter-based model uses eight discrete parameters to characterize the design space and as inputs to the model. The trained GRU model can efficiently predict the response of a new design in as little as 0.16 ms and allows rapid performance evaluation of 128000 designs in the design space. The GRU predictions identified high-performance structures, and four design trends that affect the specific energy absorption were extracted and discussed.",2307.00986v2 2023-07-07,Using electrical impedance spectroscopy to identify equivalent circuit models of lubricated contacts with complex geometry: in-situ application to mini traction machine,"Electrical contact resistance or capacitance as measured between a lubricated contact has been used in tribometers, partially reflecting the lubrication condition. In contrast, the electrical impedance provides rich information of magnitude and phase, which can be interpreted using equivalent circuit models, enabling more comprehensive measurements, including the variation of lubricant film thickness and the asperity (metal to metal) contact area. An accurate circuit model of the lubricated contact is critical as needed for the electrical impedance analysis. However, existing circuit models are hand derived and suited to interfaces with simple geometry, such as parallel plates, concentric and eccentric cylinders. Circuit model identification of lubricated contacts with complex geometry is challenging. This work takes the ball-on-disc lubricated contact in a Mini Traction Machine (MTM) as an example, where screws on the ball, grooves on the disc, and contact close to the disc edge make the overall interface geometry complicated. The electrical impedance spectroscopy (EIS) is used to capture its frequency response, with a group of load, speed, and temperature varied and tested separately. The results enable an identification of equivalent circuit models by fitting parallel resistor-capacitor models, the dependence on the oil film thickness is further calibrated using a high-accuracy optical interferometry, which is operated under the same lubrication condition as in the MTM. Overall, the proposed method is applicable to general lubricated interfaces for the identification of equivalent circuit models, which in turn facilitates in-situ tribo-contacts with electric impedance measurement of oil film thickness. It does not need transparent materials as optical techniques do, or structural modifications for piezoelectric sensor mounting as ultrasound techniques do.",2307.03668v1 2023-08-22,Magnetic Skyrmion: From Fundamental Physics to Pioneering Applications,"Skyrmionic devices exhibit energy-efficient and high-integration data storage and computing capabilities due to their small size, topological protection, and low drive current requirements. So, to realize these devices, an extensive study, from fundamental physics to practical applications, becomes essential. In this article, we present an exhaustive review of the advancements in understanding the fundamental physics behind magnetic skyrmions and the novel data storage and computing technologies based on them. We begin with an in-depth discussion of fundamental concepts such as topological protection, stability, statics and dynamics essential for understanding skyrmions, henceforth the foundation of skyrmion technologies. For the realization of CMOS-compatible skyrmion functional devices, the writing and reading of the skyrmions are crucial. We discuss the developments in different writing schemes such as STT, SOT, and VCMA. The reading of skyrmions is predominantly achieved via two mechanisms: the Magnetoresistive Tunnel Junction (MTJ) TMR effect and topological resistivity (THE). So, a thorough investigation into the Skyrmion Hall Effect, topological properties, and emergent fields is also provided, concluding the discussion on skyrmion reading developments. Based on the writing and reading schemes, we discuss the applications of the skyrmions in conventional logic, unconventional logic, memory applications, and neuromorphic computing in particular. Subsequently, we present an overview of the potential of skyrmion-hosting Majorana Zero Modes (MZMs) in the emerging Topological Quantum Computation and helicity-dependent skyrmion qubits.",2308.11811v2 2023-09-11,"Ultrafast optical properties of stoichiometric and non-stoichiometric refractory metal nitrides TiNx, ZrNx, and HfNx","Refractory metal nitrides have recently gained attention in various fields of modern photonics due to their cheap and robust production technology, silicon-technology compatibility, high thermal and mechanical resistance, and competitive optical characteristics in comparison to typical plasmonic materials like gold and silver. In this work, we demonstrate that by varying the stoichiometry of sputtered nitride films, both static and ultrafast optical responses of refractory metal nitrides can efficiently be controlled. We further prove that the spectral changes in ultrafast transient response are directly related to the position of the epsilon-near-zero region. At the same time, the analysis of the temporal dynamics allows us to identify three time components - the ""fast"" femtosecond one, the ""moderate"" picosecond one, and the ""slow"" at the nanosecond time scale. We also find out that the non-stoichiometry does not significantly decrease the recovery time of the reflectance value. Our results show the strong electron-phonon coupling and reveal the importance of both the electron and lattice temperature-induced changes in the permittivity near the ENZ region and the thermal origin of the long tail in the transient optical response of refractory nitrides.",2309.05593v1 2023-10-01,Effect of Spin Fluctuations on Magnetoresistance and Anomalous Hall Effect in the Chiral Magnet Co8Zn8Mn4,"The beta Mn type Co-Zn-Mn alloys have seized significant attention due to their ability to host skyrmions at room temperature. Here we analyse the unconventional magneto-transport properties of Co8Zn8Mn4 single crystals with a Curie temperature of 275 K. A negative magnetoresistance is obtained over a wide temperature range of 50K to 300K. The deviation of the isothermal magnetoresistance (MR) curves from linearity to non-linearity as one approaches higher temperatures points towards the transition from the dominance of magnons to spin fluctuations. In the paramagnetic phase, the change in the shape of the MR curve has been explained using the Khosla and Fischer model. The relationship between the anomalous Hall effect (AHE) and longitudinal resistivity reveals the dominance of the skew-scattering mechanism, which is inexplicable based on the theories of semi-classical magneto-transport. We experimentally determine that the spin fluctuation is the source of the skew-scattering mechanism in Co8Zn8Mn4. In general skew-scattering mechanisms predominate in compounds with high conductivity, but our findings demonstrate that this is not always the case and that other aspects also require equal consideration. Our work throws new light on the predominant scattering mechanism in chiral magnets with skyrmionics phase at low conductivity.",2310.00739v1 2023-11-01,Annealing effects on the magnetic and magnetotransport properties of iron oxide nanoparticles self-assemblies,"In magnetic tunnel junctions based on iron oxide nanoparticles the disorder and the oxidation state of the surface spin as well as the nanoparticles functionalization play a crucial role in the magnetotransport properties. In this work, we report a systematic study of the effects of vacuum annealing on the structural, magnetic and transport properties of self-assembled ~10 nm Fe3O4 nanoparticles. The high temperature treatment (from 573 to 873 K) decomposes the organic coating into amorphous carbon, reducing the electrical resistivity of the assemblies by 4 orders of magnitude. At the same time, the 3Fe2+/(Fe3++Fe2+) ratio is reduced from 1.11 to 0.13 when the annealing temperature of the sample increases from 573 to 873 K, indicating an important surface oxidation. Although the 2 nm physical gap remains unchanged with the thermal treatment, a monotonous decrease of tunnel barrier width was obtained from the electron transport measurements when the annealing temperature increases, indicating an increment in the number of defects and hot-spots in the gap between the nanoparticles. This is reflected in the reduction of the spin dependent tunneling, which reduces the interparticle magnetoresistance. This work shows new insights about influence of the nanoparticle interfacial composition, as well their the spatial arrangement, on the tunnel transport of self-assemblies, and evidence the importance of optimizing the nanostructure fabrication for increasing the tunneling current without degrading the spin polarized current.",2311.00700v1 2023-11-08,Incorporating temporal dynamics of mutations to enhance the prediction capability of antiretroviral therapy's outcome for HIV-1,"Motivation: In predicting HIV therapy outcomes, a critical clinical question is whether using historical information can enhance predictive capabilities compared with current or latest available data analysis. This study analyses whether historical knowledge, which includes viral mutations detected in all genotypic tests before therapy, their temporal occurrence, and concomitant viral load measurements, can bring improvements. We introduce a method to weigh mutations, considering the previously enumerated factors and the reference mutation-drug Stanford resistance tables. We compare a model encompassing history (H) with one not using it (NH). Results: The H-model demonstrates superior discriminative ability, with a higher ROC-AUC score (76.34%) than the NH-model (74.98%). Significant Wilcoxon test results confirm that incorporating historical information improves consistently predictive accuracy for treatment outcomes. The better performance of the H-model might be attributed to its consideration of latent HIV reservoirs, probably obtained when leveraging historical information. The findings emphasize the importance of temporal dynamics in mutations, offering insights into HIV infection complexities. However, our result also shows that prediction accuracy remains relatively high even when no historical information is available. Supplementary information: Supplementary material is available.",2311.04846v1 2024-03-12,Fragmentation of Dense Rotation-Dominated Structures Fed by Collapsing Gravomagneto-Sheetlets and Origin of Misaligned 100 au-Scale Binaries and Multiple Systems,"The majority of stars are in binary/multiple systems. How such systems form in turbulent, magnetized cores of molecular clouds in the presence of non-ideal MHD effects remains relatively under-explored. Through ATHENA++-based non-ideal MHD AMR simulations with ambipolar diffusion, we show that the collapsing protostellar envelope is dominated by dense gravomagneto-sheetlets, a turbulence-warped version of the classic pseuodisk produced by anisotropic magnetic resistance to the gravitational collapse, in agreement with previous simulations of turbulent, magnetized single-star formation. The sheetlets feed mass, magnetic fields, and angular momentum to a Dense ROtation-Dominated (DROD) structure, which fragments into binary/multiple systems. This DROD fragmentation scenario is a more dynamic variant of the traditional disk fragmentation scenario for binary/multiple formation, with dense spiral filaments created by inhomogeneous feeding from the highly structured larger-scale sheetlets rather than the need for angular momentum transport, which is dominated by magnetic braking. Collisions between the dense spiraling filaments play a key role in pushing the local magnetic Toomre parameter $Q_\mathrm{m}$ below unity, leading to gravitational collapse and stellar companion formation provided that the local material is sufficiently demagnetized, with a plasma-$\beta$ of order unity or more. This mechanism can naturally produce {\it in situ} misaligned systems on the 100-au scale, often detected with high-resolution ALMA observations. Our simulations also highlight the importance of non-ideal MHD effects, which affect whether fragmentation occurs and, if so, the masses and orbital parameters of the stellar companions formed.",2403.07777v1 2024-03-17,Thickness effect on superconducting properties of niobium films for radio-frequency cavity applications,"Niobium-coated copper radio-frequency cavities are cost-effective alternatives to bulk niobium cavities, given the lower material costs of copper substrates and their operation in liquid helium at around 4.2 K. However, these cavities historically exhibited a gradual degradation in performance with the accelerating field. This phenomenon, not yet fully understood, limits the application of niobium thin film cavities in accelerators where the real-estate gradient needs to be maximized. Recent studies on niobium films deposited on copper using high power impulse magnetron sputtering (HiPIMS) technique show promising results in mitigating the performance degradation of niobium thin film radio-frequency cavities. This paper examines the effect of film thickness on the superconducting properties of niobium films deposited on copper using HiPIMS. The study provides insights into how the critical temperature, transition width, lower and upper critical fields, and critical current density vary with the film thickness. Increasing the thickness of niobium films deposited through HiPIMS is found to enhance superconducting properties and reduce densities of defects and structural irregularities in the crystalline lattice. This shows potential for enhancing overall performance and potentially mitigating the observed performance degradation in niobium thin film radio-frequency cavities. Additionally, the Ivry's scaling relation among critical temperature, thickness, and sheet resistance at the normal state appears applicable to niobium films up to approximately 4 $\mu$m. This extends the previously confirmed validity for niobium films, which was limited to around 300 nm thickness.",2403.11245v1 2024-04-15,Stiffness-Tuneable Limb Segment with Flexible Spine for Malleable Robots,"Robotic arms built from stiffness-adjustable, continuously bending segments serially connected with revolute joints have the ability to change their mechanical architecture and workspace, thus allowing high flexibility and adaptation to different tasks with less than six degrees of freedom, a concept that we call malleable robots. Known stiffening mechanisms may be used to implement suitable links for these novel robotic manipulators; however, these solutions usually show a reduced performance when bending due to structural deformation. By including an inner support structure this deformation can be minimised, resulting in an increased stiffening performance. This paper presents a new multi-material spine-inspired flexible structure for providing support in stiffness-controllable layer-jamming-based robotic links of large diameter. The proposed spine mechanism is highly movable with type and range of motions that match those of a robotic link using solely layer jamming, whilst maintaining a hollow and light structure. The mechanics and design of the flexible spine are explored, and a prototype of a link utilising it is developed and compared with limb segments based on granular jamming and layer jamming without support structure. Results of experiments verify the advantages of the proposed design, demonstrating that it maintains a constant central diameter across bending angles and presents an improvement of more than 203% of resisting force at 180 degrees.",2404.09653v1 2024-04-23,Ultrafast nanocomposite scintillators based on Cd-enhanced CsPbCl3 nanocrystals in polymer matrix,"Lead halide perovskite nanocrystals (LHP-NCs) embedded in polymer matrices are gaining traction for next-generation radiation detectors. While progress has been made on green-emitting CsPbBr3 NCs, scant attention has been given to the scintillation properties of CsPbCl3 NCs, which emit size-tunable UV-blue light matching the peak efficiency of ultrafast photodetectors. In this study, we explore the scintillation characteristics of CsPbCl3 NCs produced through a scalable method and treated with CdCl2. Spectroscopic, radiometric and theoretical analysis on both untreated and treated NCs uncover deep hole trap states due to surface undercoordinated chloride ions, eliminated by Pb to Cd substitution. This yields near-perfect efficiency and resistance to polyacrylate mass-polymerization. Radiation hardness tests demonstrate stability to high gamma doses while time-resolved experiments reveal ultrafast radioluminescence with an average lifetime as short as 210 ps. These findings enhance our comprehension of LHP NCs' scintillation properties, positioning CsPbCl3 as a promising alternative to conventional fast scintillators.",2404.14813v1 1994-10-19,"$Pb_{0.4}Bi_{1.6}Sr_{2}Ca_{1}Cu_{2}O_{8+x}$ and Oxygen Stoichiometry: Structure, Resistivity, Fermi Surface Topology and Normal State Properties","$Pb_{0.4}Bi_{1.6}Sr_2CaCu_2O_{8+x}$ ($Bi(Pb)-$2212) single crystal samples were studied using transmission electron microscopy (TEM), $ab-$plane ($\rho_{ab}$) and $c-$axis ($\rho_c$) resistivity, and high resolution angle-resolved ultraviolet photoemission spectroscopy (ARUPS). TEM reveals that the modulation in the $b-$axis for $Pb(0.4)-$doped $Bi(Pb)-$2212 is dominantly of $Pb-$type that is not sensitive to the oxygen content of the system, and the system clearly shows a structure of orthorhombic symmetry. Oxygen annealed samples exhibit a much lower $c-$axis resistivity and a resistivity minimum at $80-130$K. He-annealed samples exhibit a much higher $c-$axis resistivity and $d\rho_c/dT<0$ behavior below 300K. The Fermi surface (FS) of oxygen annealed $Bi(Pb)-$2212 mapped out by ARUPS has a pocket in the FS around the $\bar{M}$ point and exhibits orthorhombic symmetry. There are flat, parallel sections of the FS, about 60\% of the maximum possible along $k_x = k_y$, and about 30\% along $k_x = - k_y$. The wavevectors connecting the flat sections are about $0.72(\pi, \pi)$ along $k_x = k_y$, and about $0.80(\pi, \pi)$ along $k_x = - k_y$, rather than $(\pi,\pi)$. The symmetry of the near-Fermi-energy dispersing states in the normal state changes between oxygen-annealed and He-annealed samples.",9410069v1 2003-05-30,General expressions for the electrical resistivity and thermal conductivity of twinned crystals,"General expressions are derived for the electrical resisitivity and thermal conductivity of a twinned single crystal. Particular attention is paid to the effect of the structure of the twin domains on these transport coefficients. Edge effects are also considered. The expression for the thermal conductivity is used to fit data for a twinned single crystal of 0.8% Zn-doped YBa2Cu3O6.98. The expression for the electrical resistivity is used to fit previously published electrical resistivity data for a twinned single crystal of YBa2Cu3O6.9. It is found that twin boundaries are not a significant source of electron scattering in high-quality single crystals of Y-123. We cannot rule out scattering of phonons by twin boundaries in these crystals, with up to 12% suppression of the phonon component of the thermal conductivity. The related problem of determining the electrical resistivity and thermal conductivity of a crystal with oblique and alternating isotropic regions of different conductivities is also solved.",0305698v5 2003-06-13,Behavior of the contacts of Quantum Hall Effect devices at high currents : an electronic thermometer,"This paper reports on an experimental study of the contact resistance of Hall bars in the Quantum Hall Effect regime while increasing the current through the sample. These measurements involve also the longitudinal resistance and they have been always performed before the breakdown of the Quantum Hall Effect. Our investigations are restricted to the $i=2$ plateau which is used in all metrological measurements of the von Klitzing constant $R_K$. A particular care has been taken concerning the configuration of the measurement. Four configurations were used for each Hall bar by reversing the current and the magnetic field polarities. Several samples with different width have been studied and we observed that the critical current for the contact resistance increases with the width of the Hall bar as previously observed for the critical current of the longitudinal resistance. The critical currents exhibit either a linear or a sublinear increase. All our observations are interpreted in the current understanding of the Quantum hall effect brekdown. Our analysis suggests that a heated region appears at the current contact, develops and then extends in the whole sample while increasing the current. Consequently, we propose to use the contact resistance as an electronic thermometer for the Hall fluid.",0306368v3 2004-07-19,Resistivity studies under hydrostatic pressure on a low-resistance variant of the quasi-2D organic superconductor kappa-(BEDT-TTF)2Cu[N(CN)2]Br: quest for intrinsic scattering contributions,"Resistivity measurements have been performed on a low (LR)- and high (HR)-resistance variant of the kappa-(BEDT-TTF)_2Cu[N(CN)_2]Br superconductor. While the HR sample was synthesized following the standard procedure, the LR crystal is a result of a somewhat modified synthesis route. According to their residual resistivities and residual resistivity ratios, the LR crystal is of distinctly superior quality. He-gas pressure was used to study the effect of hydrostatic pressure on the different transport regimes for both variants. The main results of these comparative investigations are (i) a significant part of the inelastic-scattering contribution, which causes the anomalous rho(T) maximum in standard HR crystals around 90 K, is sample dependent, i.e. extrinsic in nature, (ii) the abrupt change in rho(T) at T* approx. 40 K from a strongly temperature-dependent behavior at T > T* to an only weakly T-dependent rho(T) at T < T* is unaffected by this scattering contribution and thus marks an independent property, most likely a second-order phase transition, (iii) both variants reveal a rho(T) proportional to AT^2 dependence at low temperatures, i.e. for T_c < T < T_0, although with strongly sample-dependent coefficients A and upper bounds for the T^2 behavior measured by T_0. The latter result is inconsistent with the T^2 dependence originating from coherent Fermi-liquid excitations.",0407478v1 2004-10-28,Transport properties in manganite thin films,"The resistivity of thin $La_{0.7}A_{0.3}MnO_{3}$ films ($A=Ca, Sr$) is investigated in a wide temperature range. The comparison of the resistivities is made among films grown by different techniques and on several substrates allowing to analyze samples with different amounts of disorder. In the low-temperature nearly half-metallic ferromagnetic state the prominent contribution to the resistivity scales as $T^{\alpha}$ with $\alpha \simeq 2.5$ for intermediate strengths of disorder supporting the theoretical proposal of single magnon scattering in presence of minority spin states localized by the disorder. For large values of disorder the low-temperature behavior of the resistivity is well described by the law $T^{3}$ characteristic of anomalous single magnon scattering processes, while in the regime of low disorder the $\alpha$ exponent tends to a value near 2. In the high temperature insulating paramagnetic phase the resistivity shows the activated behavior characteristic of polaronic carriers. Finally in the whole range of temperatures the experimental data are found to be consistent with a phase separation scenario also in films doped with strontium ($A=Sr$).",0410743v1 2008-12-22,Joule Heating and Anomalous Resistivity in the Solar Corona,"Recent radioastronomical observations of Faraday rotation in the solar corona can be interpreted as evidence for coronal currents, with values as large as $2.5 \times 10^9$ Amperes (Spangler 2007). These estimates of currents are used to develop a model for Joule heating in the corona. It is assumed that the currents are concentrated in thin current sheets, as suggested by theories of two dimensional magnetohydrodynamic turbulence. The Spitzer result for the resistivity is adopted as a lower limit to the true resistivity. The calculated volumetric heating rate is compared with an independent theoretical estimate by Cranmer et al (2007). This latter estimate accounts for the dynamic and thermodynamic properties of the corona at a heliocentric distance of several solar radii. Our calculated Joule heating rate is less than the Cranmer et al estimate by at least a factor of $3 \times 10^5$. The currents inferred from the observations of Spangler (2007) are not relevant to coronal heating unless the true resistivity is enormously increased relative to the Spitzer value. However, the same model for turbulent current sheets used to calculate the heating rate also gives an electron drift speed which can be comparable to the electron thermal speed, and larger than the ion acoustic speed. It is therefore possible that the coronal current sheets are unstable to current-driven instabilities which produce high levels of waves, enhance the resistivity and thus the heating rate.",0812.4220v1 2009-06-24,Turbulent resistivity driven by the magnetorotational instability,"We measure the turbulent resistivity in the nonlinear regime of the MRI, and evaluate the turbulent magnetic Prandtl number. We perform a set of numerical simulations with the Eulerian finite volume codes Athena and Ramses in the framework of the shearing box model. We consider models including explicit dissipation coefficients and magnetic field topologies such that the net magnetic flux threading the box in both the vertical and azimuthal directions vanishes. We first demonstrate good agreement between the two codes by comparing the properties of the turbulent states in simulations having identical microscopic diffusion coefficients (viscosity and resistivity). We find the properties of the turbulence do not change when the box size is increased in the radial direction, provided it is elongated in the azimuthal direction. To measure the turbulent resistivity in the disk, we impose a fixed electromotive force on the flow and measure the amplitude of the saturated magnetic field that results. We obtain a turbulent resistivity that is in rough agreement with mean field theories like the Second Order Smoothing Approximation. The numerical value translates into a turbulent magnetic Prandtl number Pm_t of order unity. Pm_t appears to be an increasing function of the forcing we impose. It also becomes smaller as the box size is increased in the radial direction, in good agreement with previous results obtained in very large boxes. Our results are in general agreement with other recently published papers studying the same problem but using different methodology. Thus, our conclusion that Pm_t is of order unity appears robust.",0906.4422v2 2009-07-08,Turbulent resistivity evaluation in MRI generated turbulence,"(abriged) MRI turbulence is a leading mechanism for the generation of an efficient turbulent transport of angular momentum in an accretion disk through a turbulent viscosity effect. It is believed that the same process could also transport large-scale magnetic fields in disks, reshaping the magnetic structures in these objects. This process, known as turbulent resistivity, has been suggested and used in several accretion-ejection models and simulations to produce jets. Still, the efficiency of MRI-driven turbulence to transport large-scale magnetic fields is largely unknown. We investigate this problem both analytically and numerically. We introduce a linear calculation of the MRI in the presence of a spatially inhomogeneous mean magnetic field. We show that, in this configuration, MRI modes lead to an efficient magnetic field transport, on the order of the angular momentum transport. We next use fully non linear simulations of MRI turbulence to compute the turbulent resistivity in several magnetic configurations. We find that the turbulent resistivity is on the order of the turbulent viscosity in all our simulations, although somewhat lower. The turbulent resistivity tensor is found to be highly anisotropic with a diffusion coefficient 3 times greater in the radial direction than in the vertical direction. These results support the possibility of driving jets from turbulent disks; the resulting jets may not be steady.",0907.1393v1 2009-07-15,Transport properties and the anisotropy of Ba_{1-x}K_xFe_2As_2 single crystals in normal and superconducting states,"The transport and superconducting properties of Ba_{1-x}K_xFe_2As_2 single crystals with T_c = 31 K were studied. Both in-plane and out-of plane resistivity was measured by modified Montgomery method. The in-plane resistivity for all studied samples, obtained in the course of the same synthesis, is almost the same, unlike to the out-of plane resistivity, which differ considerably. We have found that the resistivity anisotropy \gamma=\rho_c /\rho_{ab} is almost temperature independent and lies in the range 10-30 for different samples. This, probably, indicates on the extrinsic nature of high out-of-plane resistivity, which may appear due to the presence of the flat defects along Fe-As layers in the samples. This statement is supported by comparatively small effective mass anisotropy, obtained from the upper critical field measurements, and from the observation of the so-called ""Friedel transition"", which indicates on the existence of some disorder in the samples in c-direction.",0907.2598v1 2010-12-31,In-plane anisotropy of electrical resistivity in the strain-detwinned SrFe2As2,"Intrinsic, in-plane anisotropy of electrical resistivity was studied on mechanically detwinned single crystals of SrFe$_2$As$_2$ above and below the temperature of the coupled structural/magnetic transition, $T_{\textrm{TO}}$. Resistivity is smaller for electrical current flow along the orthorhombic $a_o$ direction (direction of antiferromagnetically alternating magnetic moments) and is larger for transport along the $b_o$ direction (direction of ferromagnetic chains), which is similar to CaFe$_2$As$_2$ and BaFe$_2$As$_2$ compounds. A strongly first order structural transition in SrFe$_2$As$_2$ was confirmed by high-energy x-ray measurements, with the transition temperature, and character unaffected by moderate strain. For small strain levels, which are just sufficient to detwin the sample, we find a negligible effect on the resistivity above $T_{\textrm{TO}}$. With the increase of strain, the resistivity anisotropy starts to develop above $T_{\textrm{TO}}$, clearly showing the relation of anisotropy to an anomalously strong response to strain. Our study suggests that electronic nematicity cannot be observed in the FeAs based compounds in which the structural transition is strongly first order.",1101.0274v1 2012-12-05,Electric field driven destabilization of the insulating state in nominally pure LaMnO3,"We report an electric field driven destabilization of the insulating state in nominally pure LaMnO3 single crystal with a moderate field which leads to a resistive state transition below 300 K. The transition is between the insulating state in LaMnO3 and a high resistance bad metallic state that has a temperature independent resistivity. The transition occurs at a threshold field (Eth) which shows a steep enhancement on cooling. While at lower temperatures the transition is sharp and involves large change in resistance but it softens on heating and eventually absent above 280K. When the Mn4+ content is increased by Sr substitution up to x=0.1, the observed transition though observable in certain temperature range, softens considerably. The observation has been explained as bias driven percolation type transition between two coexisting phases, where the majority phase is a charge and orbitally ordered polaronic insulating phase and the minority phase is a bad metallic phase. The mobile fraction f of the bad metallic phase deduced from the experimental data follows an activated kinetics with the activation energy nearly equal to 200 meV and the prefactor fo is a strong function of the field that leads to a rapid enhancement of f on application of field leading to the resistive state transition. We suggest likely scenarios for such co-existing phases in nominally pure LaMnO3 that can lead to the bias driven percolation type transition.",1212.1001v2 2013-09-21,A switch to reduce resistivity in smoothed particle magnetohydrodynamics,"Artificial resistivity is included in Smoothed Particle Magnetohydrodynamics simulations to capture shocks and discontinuities in the magnetic field. Here we present a new method for adapting the strength of the applied resistivity so that shocks are captured but the dissipation of the magnetic field away from shocks is minimised. Our scheme utilises the gradient of the magnetic field as a shock indicator, setting {\alpha}_B = h|gradB|/|B|, such that resistivity is switched on only where strong discontinuities are present. The advantage to this approach is that the resistivity parameter does not depend on the absolute field strength. The new switch is benchmarked on a series of shock tube tests demonstrating its ability to capture shocks correctly. It is compared against a previous switch proposed by Price & Monaghan (2005), showing that it leads to lower dissipation of the field, and in particular, that it succeeds at capturing shocks in the regime where the Alfv\'en speed is much less than the sound speed (i.e., when the magnetic field is very weak). It is also simpler. We also demonstrate that our recent constrained divergence cleaning algorithm has no difficulty with shock tube tests, in contrast to other implementations.",1309.5437v1 2013-10-04,Piggyback resistive Micromegas,"Piggyback Micromegas consists in a novel readout architecture where the anode element is made of a resistive layer on a ceramic substrate. The resistive layer is deposited on the thin ceramic substrate by an industrial process which provides large dynamic range of resistivity (10$^6$ to 10$^{10}$\,M$\Omega$/square). The particularity of this new structure is that the active part is entirely dissociated from the read-out element. This gives a large flexibility on the design of the anode structure and the readout scheme. Without significant loss, signals are transmitted by capacitive coupling to the read-out pads. The detector provides high gas gain, good energy resolution and the resistive layer assures spark protection for the electronics. This assembly could be combined with modern pixel array electronic ASICs. First tests with different Piggyback detectors and configurations will be presented. This structure is adequate for cost effective fabrication and low outgassing detectors. It was designed to perform in sealed mode and its long term stability has been extensively studied. In addition perspectives on the future developments will be evoked.",1310.1242v1 2013-10-15,Recent advances with THGEM detectors,"The Thick Gaseous Electron Multiplier (THGEM) is a simple and robust electrode suitable for large area detectors. In this work the results of extensive comparative studies of the physical properties of different THGEM-based structures are reviewed. The focus is on newly suggested THGEM-like WELL configurations as well as on recently developed characterization methods. The WELL structures are single-sided THGEM electrodes directly coupled to different anode readout electrodes. The structures differ by the coupling concept of the bottom THGEM electrode to the metallic readout pads: a Thick WELL (THWELL) with direct coupling; the Resistive WELL (RWELL) and the Segmented Resistive WELL (SRWELL) coupled through thin resistive films deposited on insulating sheets and a Resistive-Plate WELL (RPWELL) coupled through a plate of high bulk resistivity. The results are compared to that of traditional double-sided THGEM electrodes followed by induction gaps - in some cases with moderate additional multiplication within the gap. We compare the different configurations in terms of gain, avalanche extension, discharge-rate and magnitude as well as rate capabilities over a broad dynamic range - exploiting a method that mimics highly ionizing particles in the laboratory. We report on recent studies of avalanche distribution in THGEM holes using optical readout.",1310.3912v1 2014-10-10,"On the bad metallicity and phase diagrams of Fe$_{1+δ}X$ ($X$ =Te, Se, S, solid solutions): an electrical resistivity study","Based on a systematic analysis of the thermal evolution of the resistivities of Fe-based chalcogenides Fe$_{1+\delta }$Te$_{1-x}X_{x}$ ($X$= Se, S), it is inferred that their often observed nonmetallic resistivities are related to a presence of two resistive channels: one is a high-temperature thermally-activated process while the other is a low-temperature log-in-$T$ process. On lowering temperature, there are often two metal-to-nonmetall crossover events: one from the high-$T$ thermally-activated nonmetallic regime into a metal-like phase and the other from the log-in-$T$ regime into a second metal-like phase. Based on these events, together with the magnetic and superconducting transitions, a phase diagram is constructed for each series. We discuss the origin of both processes as well as the associated crossover events. We also discuss how these resistive processes are being influenced by pressure, intercalation, disorder, doping, or sample condition and, in turn, how these modifications are shaping the associated phase diagrams.",1410.2676v1 2016-11-17,On the measurements of numerical viscosity and resistivity in Eulerian MHD codes,"We propose a simple ansatz for estimating the value of the numerical resistivity and the numerical viscosity of any Eulerian MHD code. We test this ansatz with the help of simulations of the propagation of (magneto)sonic waves, Alfven waves, and the tearing mode instability using the MHD code Aenus. By comparing the simu- lation results with analytical solutions of the resistive-viscous MHD equations and an empirical ansatz for the growth rate of tearing modes we measure the numerical viscosity and resistivity of Aenus. The comparison shows that the fast-magnetosonic speed and wavelength are the characteristic velocity and length, respectively, of the aforementioned (relatively simple) systems. We also determine the dependance of the numerical viscosity and resistivity on the time integration method, the spatial reconstruction scheme and (to a lesser extent) the Riemann solver employed in the simulations. From the measured results we infer the numerical resolution (as a function of the spatial reconstruction method) required to properly resolve the growth and saturation level of the magnetic field amplified by the magnetorotational instability in the post-collapsed core of massive stars. Our results show that it is to the best advantage to resort to ultra-high order methods (e.g., 9th-order Monotonicity Preserving method) to tackle this problem properly, in particular in three dimensional simulations.",1611.05858v2 2017-02-06,Rings and gaps produced by variable magnetic disk winds and avalanche accretion streams: I. Axisymmetric resistive MHD simulations,"Rings and gaps are being observed in an increasing number of disks around young stellar objects. We illustrate the formation of such radial structures through idealized, 2D (axisymmetric) resistive MHD simulations of coupled disk-wind systems threaded by a relatively weak poloidal magnetic field (plasma-$\beta \sim 10^3$). We find two distinct modes of accretion depending on the resistivity and field strength. A small resistivity or high field strength promotes the development of rapidly infalling `avalanche accretion streams' in a vertically extended disk envelope that dominates the dynamics of the system, especially the mass accretion. The streams are suppressed in simulations with larger resistivities or lower field strengths, where most of the accretion instead occurs through a laminar disk. In these simulations, the disk accretion is driven mainly by a slow wind that is typically accelerated by the pressure gradient from a predominantly toroidal magnetic field. Both wind-dominated and stream-dominated modes of accretion create prominent features in the surface density distribution of the disk, including rings and gaps, with a strong spatial variation of the magnetic flux relative to the mass. Regions with low mass-to-flux ratios accrete quickly, leading to the development of gaps, whereas regions with higher mass-to-flux ratios tend to accrete more slowly, allowing matter to accumulate and form dense rings. In some cases, avalanche accretion streams are observed to produce dense rings directly through continuous feeding. We discuss the implications of ring and gap formation driven by winds and streams on grain growth and planet formation.",1702.01565v2 2017-09-18,Log-rise of the Resistivity in the Holographic Kondo Model,"We study a single-channel Kondo effect using a recently developed holographic large-$N$ technique. In order to obtain resistivity of this model, we introduce a probe field. The gravity dual of a localized fermionic impurity in 1+1-dimensional host matter is constructed by embedding a localized 2-dimensional Anti-de Sitter (\ads{2})-brane in the bulk of \ads{3}. This helps us construct an impurity charge density which acts as a source to the bulk equation of motion of the probe gauge field. The functional form of the charge density is obtained independently by solving the equations of motion for the fields confined to the \ads{2}-brane. The asymptotic solution of the probe field is dictated by the impurity charge density, which in turn, affects the current-current correlation functions, and hence the resistivity. Our choice of parameters tunes the near-boundary impurity current to be marginal, resulting in a $\log T$ behavior in the UV resistivity, as is expected for the Kondo problem. The resistivity at the IR fixed point turns out to be zero, signaling a complete screening of the impurity.",1709.06086v2 2019-07-11,First results of Resistive-Plate Well (RPWELL) detector operation at 163 K,"We present for the first time, discharge-free operation at cryogenic conditions of a Resistive-Plate WELL (RPWELL) detector. It is a single-sided Thick Gaseous Electron Multiplier (THGEM) coupled to a readout anode via a plate of high bulk resistivity. The results of single- and double-stage RPWELL detectors operated in stable conditions in Ne/5$\%$CH$_{4}$ at 163 K are summarized. The RPWELL comprised a ferric-based (Fe$^{3+}$) ceramic composite (""Fe-ceramic"") as the resistive plate, of volume resistivity $\sim$$10^{11}$ $\Omega$$\cdot$cm at this temperature. Gains of $\sim$$10^{4}$ and $\sim$$10^{5}$ were reached with the single-stage RPWELL, with 6 keV X-rays and single UV-photons, respectively. The double-stage detector, a THGEM followed by the RPWELL, reached gains $\sim$$10^{5}$ and $\sim$$10^{6}$ with X-rays and single UV-photons, respectively. The results were obtained with and without a CsI photocathode on the first multiplying element. Potential applications at these cryogenic conditions are discussed.",1907.05057v1 2020-04-10,Linear in temperature resistivity in the limit of zero temperature from the time reparameterization soft mode,"The most puzzling aspect of the 'strange metal' behavior of correlated electron compounds is that the linear in temperature resistivity often extends down to low temperatures, lower than natural microscopic energy scales. We consider recently proposed deconfined critical points (or phases) in models of electrons in large dimension lattices with random nearest-neighbor exchange interactions. The criticality is in the class of Sachdev-Ye-Kitaev models, and exhibits a time reparameterization soft mode representing gravity in dual holographic theories. We compute the low temperature resistivity in a large $M$ limit of models with SU($M$) spin symmetry, and find that the dominant temperature dependence arises from this soft mode. The resistivity is linear in temperature down to zero temperature at the critical point, with a co-efficient universally proportional to the product of the residual resistivity and the co-efficient of the linear in temperature specific heat. We argue that the time reparameterization soft mode offers a promising and generic mechanism for resolving the strange metal puzzle.",2004.05182v4 2017-07-31,Universal linear-temperature resistivity: possible quantum diffusion transport in strongly correlated superconductors,"The strongly correlated electron fluids in high temperature cuprate superconductors demonstrate an anomalous linear temperature ($T$) dependent resistivity behavior, which persists to a wide temperature range without exhibiting saturation. As cooling down, those electron fluids lose the resistivity and condense into the superfluid. However, the origin of the linear-$T$ resistivity behavior and its relationship to the strongly correlated superconductivity remain a mystery. Here we report a universal relation $d\rho/dT=(\mu_0k_B/\hbar)\lambda^2_L$, which bridges the slope of the linear-$T$-dependent resistivity ($d\rho/dT$) to the London penetration depth $\lambda_L$ at zero temperature among cuprate superconductor Bi$_2$Sr$_2$CaCu$_2$O$_{8+\delta}$ and heavy fermion superconductors CeCoIn$_5$, where $\mu_0$ is vacuum permeability, $k_B$ is the Boltzmann constant and $\hbar$ is the reduced Planck constant. We extend this scaling relation to different systems and found that it holds for other cuprate, pnictide and heavy fermion superconductors as well, regardless of the significant differences in the strength of electronic correlations, transport directions, and doping levels. Our analysis suggests that the scaling relation in strongly correlated superconductors could be described as a hydrodynamic diffusive transport, with the diffusion coefficient ($D$) approaching the quantum limit $D\sim\hbar/m^*$, where $m^*$ is the quasi-particle effective mass.",1707.09782v1 2019-03-28,Faster Spectral Sparsification in Dynamic Streams,"Graph sketching has emerged as a powerful technique for processing massive graphs that change over time (i.e., are presented as a dynamic stream of edge updates) over the past few years, starting with the work of Ahn, Guha and McGregor (SODA'12) on graph connectivity via sketching. In this paper we consider the problem of designing spectral approximations to graphs, or spectral sparsifiers, using a small number of linear measurements, with the additional constraint that the sketches admit an efficient recovery scheme. Prior to our work, sketching algorithms were known with near optimal $\tilde O(n)$ space complexity, but $\Omega(n^2)$ time decoding (brute-force over all potential edges of the input graph), or with subquadratic time, but rather large $\Omega(n^{5/3})$ space complexity (due to their reliance on a rather weak relation between connectivity and effective resistances). In this paper we first show how a simple relation between effective resistances and edge connectivity leads to an improved $\widetilde O(n^{3/2})$ space and time algorithm, which we show is a natural barrier for connectivity based approaches. Our main result then gives the first algorithm that achieves subquadratic recovery time, i.e. avoids brute-force decoding, and at the same time nontrivially uses the effective resistance metric, achieving $n^{1.4+o(1)}$ space and recovery time. Our main technical contribution is a novel method for `bucketing' vertices of the input graph into clusters that allows fast recovery of edges of high effective resistance: the buckets are formed by performing ball-carving on the input graph using (an approximation to) its effective resistance metric. We feel that this technique is likely to be of independent interest.",1903.12165v1 2012-06-13,Current Challenges and Perspectives in Resistive Gaseous Detectors: a manifesto from RPC 2012,"Resistive gaseous detectors can be broadly defined as those operated in conditions where virtually no field lines exist that connect any two metallic electrodes sitting at different potential. This condition can be operationally recognized as 'no gas gap being delimited by two metallic electrodes'. Since early 70's, Resistive Plate Chambers (RPCs) are the most successful implementation of this idea, that leads to fully spark-protected gaseous detectors, with solid state-like reliability at working fields beyond 100kV/cm, yet enjoying the general characteristics of gaseous detectors in terms of flexibility, optimization and customization. We present a summary of the status of the field of resistive gaseous detectors as discussed in a dedicated closing session that took place during the XI Workshop for Resistive Plate Chambers and Related Detectors celebrated in Frascati, and especially we review the perspectives and ambitions towards the XII Workshop to be celebrated in Beijing in year 2014. Due to the existence of two specific reviews ([1,2]) also at this workshop, a minimum amount of overlap was found to be unavoidable. We have realized, however, that the three works provide a look at the field from different optics, so they can be largely considered to be complementary. Contrary to the initial concerns, the overall appearance seems to be fairly round, in our opinion.",1206.2735v2 2018-12-03,Resistive evolution of toroidal field configurations and their relation to magnetic clouds,"We study the resistive evolution of a localized self-organizing magnetohydrodynamic equilibrium. In this configuration the magnetic forces are balanced by a pressure force caused by a toroidal depression in the pressure. Equilibrium is attained when this low pressure region prevents further expansion into the higher-pressure external plasma. We find that, for the parameters investigated, the resistive evolution of the structures follows a universal pattern when rescaled to resistive time. The finite resistivity causes both a decrease in the magnetic field strength and a finite slip of the plasma fluid against the static equilibrium. This slip is caused by a Pfirsch-Schl\""uter type diffusion, similar to what is seen in tokamak equilibria. The net effect is that the configuration remains in Magnetostatic equilibrium whilst it slowly grows in size. The rotational transform of the structure becomes nearly constant throughout the entire structure, and decreases according to a power law. In simulations this equilibrium is observed when highly tangled field lines relax in a high-pressure (relative to the magnetic field strength) environment, a situation that occurs when the twisted field of a coronal loop is ejected into the interplanetary solar wind. In this paper we relate this localized MHD equilibrium to magnetic clouds in the solar wind.",1812.00005v1 2019-01-24,Parylene Based Memristive Devices with Multilevel Resistive Switching for Neuromorphic Applications,"In this paper, the resistive switching and neuromorphic behavior of memristive devices based on parylene, a polymer both low-cost and safe for the human body, is comprehensively studied. The Metal/Parylene/ITO sandwich structures were prepared by means of the standard gas phase surface polymerization method with different top active metal electrodes (Ag, Al, Cu or Ti of about 500 nm thickness). These organic memristive devices exhibit excellent performance: low switching voltage (down to 1 V), large OFF/ON resistance ratio (about 10^3), retention (> 10^4 s) and high multilevel resistance switching (at least 16 stable resistive states in the case of Cu electrodes). We have experimentally shown that parylene-based memristive elements can be trained by a biologically inspired spike-timing-dependent plasticity (STDP) mechanism. The obtained results have been used to implement a simple neuromorphic network model of classical conditioning. The described advantages allow considering parylene-based organic memristors as prospective devices for hardware realization of spiking artificial neuron networks capable of supervised and unsupervised learning and suitable for biomedical applications.",1901.08667v2 2020-01-24,Metal-to-metal transition and heavy-electron state in Nd$_4$Ni$_3$O$_{10-δ}$,"The trilayer nickelate Nd$_4$Ni$_3$O$_{10-\delta}$ ($\delta \approx$ 0.15) was investigated by the measurements of x-ray diffraction, electrical resistivity, magnetic susceptibility, and heat capacity. The crystal structure data suggest a higher Ni valence in the inner perovskite-like layer. At ambient pressure the resistivity shows a jump at 162 K, indicating a metal-to-metal transition (MMT). The MMT is also characterized by a magnetic susceptibility drop, a sharp specific-heat peak, and an isotropic lattice contraction. Below $\sim$ 50 K, a resistivity upturn with a log$T$ dependence shows up, accompanying with a negative thermal expansion. External hydrostatic pressure suppresses the resistivity jump progressively, coincident with the diminution of the log$T$ behavior. The low-temperature electronic specific-heat coefficient is extracted to be $\sim$ 150 mJ K$^{-2}$ mol-fu$^{-1}$, equivalent to $\sim$ 50 mJ K$^{-2}$ mol-Ni$^{-1}$, indicating an unusual heavy-electron correlated state. The novel heavy-electron state as well as the logarithmic temperature dependence of resistivity is explained in terms of the Ni$^{3+}$ centered Kondo effect in the inner layer of the (NdNiO$_3$)$_3$ trilayers.",2001.09059v2 2021-04-07,Functional annotation of creeping bentgrass protein sequences based on convolutional neural network,"Background: Creeping bentgrass (Agrostis soionifera) is a perennial grass of Gramineae, belonging to cold season turfgrass, but has poor disease resistance. Up to now, little is known about the induced systemic resistance (ISR) mechanism, especially the relevant functional proteins, which is important to disease resistance of turfgrass. Achieving more information of proteins of infected creeping bentgrass is helpful to understand the ISR mechanism. Results: With BDO treatment, creeping bentgrass seedlings were grown, and the ISR response was induced by infecting Rhizoctonia solani. High-quality protein sequences of creeping bentgrass seedlings were obtained. Some of protein sequences were functionally annotated according to the database alignment while a large part of the obtained protein sequences was left non-annotated. To treat the non-annotated sequences, a prediction model based on convolutional neural network was established with the dataset from Uniport database in three domains to acquire good performance, especially the higher false positive control rate. With established model, the non-annotated protein sequences of creeping bentgrass were analyzed to annotate proteins relevant to disease-resistance response and signal transduction. Conclusions: The prediction model based on convolutional neural network was successfully applied to select good candidates of the proteins with functions relevant to the ISR mechanism from the protein sequences which cannot be annotated by database alignment. The waste of sequence data can be avoided, and research time and labor will be saved in further research of protein of creeping bentgrass by molecular biology technology. It also provides reference for other sequence analysis of turfgrass disease-resistance research.",2104.03139v2 2021-08-19,Resistive Hot Accretion Flows with Anisotropic Pressure,"Since the collisional mean free path of charged particles in hot accretion flows can be significantly larger than the typical length-scale of the accretion flows, the gas pressure is anisotropic to magnetic field lines. For such a large collisional mean free path, the resistive dissipation can also play a key role in hot accretion flows. In this paper, we study the dynamics of resistive hot accretion flows in the presence of anisotropic pressure. We present a set of self-similar solutions where the flow variables are assumed to be a function only of radius. Our results show that the radial and rotational velocities and the sound speed increase considerably with the strength of anisotropic pressure. The increase in infall velocity and in sound speed are more significant if the resistive dissipation is taken into account. We find that such changes depend on the field strength. Our results indicate that the resistive heating is $10\%$ of the heating by the work done by anisotropic pressure when the strength of anisotropic pressure is 0.1. This value becomes higher when the strength of anisotropic pressure reduces. The increase in disk temperature can lead to heating and acceleration of the electrons in such flows. It helps us to explain the origin of phenomena such as the flares in Galactic Center Sgr A*.",2108.09829v1 2022-05-22,First Report of Susceptibility Status of the Invasive Vector: Aedes albopictus to insecticides used in vector control in Morocco,"Aedes albopictus has been newly recorded in Agdal district at Rabat in Morocco. The establishment of this invasive mosquito could affect the public health by causing serious epidemics despite of its high nuisance in urban and sub-urban areas. Vector control is mainly based on environmental management but chemical insecticides can be used to reduce adult mosquito densities during peak periods. However, the level of susceptibility of this mosquito to insecticides has not been studied yet in Morocco. This paper reports the results of the first study conducted to monitor the insecticide resistance of adult and larva Ae. albopictus to the insecticides currently used in the vector control. The study was carried out during May-June 2018 at Rabat from the north-west of the country. Adult susceptibility tests were performed following the WHO test procedures. One organochlorate (DDT 4%), one pyrethroids (cyfluthrin 0.15%), one carbamate (bendiocarb 0.1%) and one organophosphate (fenithrothion 1%) were tested at diagnostic doses (DD). The five-fold DD of bendiocarb were also used to yield information on the intensity of mosquito adult resistance. The results of the performed susceptibility bioassay showed that the vector is susceptible to cyfluthrin and resistant to DDT, bendiocarb and fenithrothion. Larval bioassays to temephos were conducted according to WHO standard operating protocol to establish the dose-mortality relationship and deduct the LC50 and LC90 then resistance ratios. We show that larval populations of Ae. albopictus are still sensible to this insecticide. This information could help policy-makers to plan insecticide resistance management.",2205.11994v1 2023-09-15,Greedy Optimization of Resistance-based Graph Robustness with Global and Local Edge Insertions,"The total effective resistance, also called the Kirchhoff index, provides a robustness measure for a graph $G$. We consider two optimization problems of adding $k$ new edges to $G$ such that the resulting graph has minimal total effective resistance (i.e., is most robust) -- one where the new edges can be anywhere in the graph and one where the new edges need to be incident to a specified focus node. The total effective resistance and effective resistances between nodes can be computed using the pseudoinverse of the graph Laplacian. The pseudoinverse may be computed explicitly via pseudoinversion; yet, this takes cubic time in practice and quadratic space. We instead exploit combinatorial and algebraic connections to speed up gain computations in an established generic greedy heuristic. Moreover, we leverage existing randomized techniques to boost the performance of our approaches by introducing a sub-sampling step. Our different graph- and matrix-based approaches are indeed significantly faster than the state-of-the-art greedy algorithm, while their quality remains reasonably high and is often quite close. Our experiments show that we can now process larger graphs for which the application of the state-of-the-art greedy approach was impractical before.",2309.08271v1 2024-05-28,Differential Voltage Analysis and Patterns in Parallel-Connected Pairs of Imbalanced Cells,"Diagnosing imbalances in capacity and resistance within parallel-connected cells in battery packs is critical for battery management and fault detection, but it is challenging given that individual currents flowing into each cell are often unmeasured. This work introduces a novel method useful for identifying imbalances in capacity and resistance within a pair of parallel-connected cells using only voltage and current measurements from the pair. Our method utilizes differential voltage analysis (DVA) when the pair is under constant current discharge and demonstrates that features of the pair's differential voltage curve (dV/dQ), namely its mid-to-high SOC dV/dQ peak's height and skewness, are sensitive to imbalances in capacity and resistance. We analyze and explain how and why these dV/dQ peak shape features change in response to these imbalances, highlighting that the underlying current imbalance dynamics resulting from these imbalances contribute to these changes. Ultimately, we demonstrate that dV/dQ peak shape features can identify the product of capacity imbalance and resistance imbalance, but cannot uniquely identify the imbalances. This work lays the groundwork for identifying imbalances in capacity and resistance in parallel-connected cell groups in battery packs, where commonly only a single current sensor is placed for each parallel cell group.",2405.17754v1 2018-02-05,Electrical-current-induced magnetic hysteresis in self-assembled vertically aligned La_{2/3}Sr_{1/3}MnO_3:ZnO-nanopillar composites,"Magnetoresistive random-access memory (MRAM) is poised to become a next-generation information storage device. Yet, many materials challenges remain unsolved before it can become a widely used memory storage solution. Among them, an urgent need is to identify a material system that is suitable for downscaling and is compatible with low-power logic applications. Self-assembled, vertically-aligned La_{2/3}Sr_{1/3}MnO_3:ZnO nanocomposites, in which La_{2/3}Sr_{1/3}MnO_3 (LSMO) matrix and ZnO nanopillars form an intertwined structure with coincident-site-matched growth occurring between the LSMO and ZnO vertical interfaces, may offer new MRAM applications by combining their superior electric, magnetic (B), and optical properties. In this paper, we show the results of electrical current induced magnetic hysteresis in magneto-resistance measurements in these nano-pillar composites. We observe that when the current level is low, for example, 1 uA, the magneto-resistance displays a linear, negative, non-hysteretic B field dependence. Surprisingly, when a large current is used, I > 10 uA, a hysteretic behavior is observed when the B field is swept in the up and down directions. This hysteresis weakens as the sample temperature is increased. A possible spin-valve mechanism related to this electrical current induced magnetic hysteresis is proposed and discussed.",1802.01632v1 2018-03-05,Measurement of Elastoresistivity at Finite Frequency by Amplitude Demodulation,"Elastoresistivity, the relation between resistivity and strain, can elucidate subtle properties of the electronic structure of a material and is an increasingly important tool for the study of strongly correlated materials. To date, elastoresistivity measurements have been predominantly performed with quasi-static (DC) strain. In this work, we demonstrate a method for using AC strain in elastoresistivity measurements. A sample experiencing AC strain has a time-dependent resistivity, which modulates the voltage produced by an AC current; this effect produces time-dependent variations in resisitivity that are directly proportional to the elastoresistivity, and which can be measured more quickly, with less strain on the sample, and with less stringent requirements for temperature stability than the previous DC technique. Example measurements between 10 Hz and 3 kHz are performed on a material with a large, well-characterized and temperature dependent elastoresistivity: the representative iron-based superconductor BaFe$_{1.975}$Co$_{0.025}$As$_2$. These measurements yield a frequency independent elastoresistivity and reproduce results from previous DC elastoresistivity methods to within experimental accuracy. We emphasize that the dynamic (AC) elastoresistivity is a distinct material-specific property that has not previously been considered.",1803.01909v2 2020-03-26,Fermi liquid behavior and colossal magnetoresistance in layered MoOCl2,"A characteristic of a Fermi liquid is the T^2 dependence of its resistivity, sometimes referred to as the Baber law. However, for most metals, this behavior is only restricted to very low temperatures, usually below 20 K. Here, we experimentally demonstrate that for the single-crystal van der Waals layered material MoOCl2, the Baber law holds in a wide temperature range up to ~120 K, indicating that the electron-electron scattering plays a dominant role in this material. Combining with the specific heat measurement, we find that the modified Kadowaki-Woods ratio of the material agrees well with many other strongly correlated metals. Furthermore, in the magneto-transport measurement, a colossal magneto-resistance is observed, which reaches ~350% at 9 T and displays no sign of saturation. With the help of first-principles calculations, we attribute this behavior to the presence of open orbits on the Fermi surface. We also suggest that the dominance of electron-electron scattering is related to an incipient charge density wave state of the material. Our results establish MoOCl2 as a strongly correlated metal and shed light on the underlying physical mechanism, which may open a new path for exploring the effects of electron-electron interaction in van der Waals layered structures.",2003.11905v1 2020-04-06,Microscopic Relaxation Channels in Materials for Superconducting Qubits,"Despite mounting evidence that materials imperfections are a major obstacle to practical applications of superconducting qubits, connections between microscopic material properties and qubit coherence are poorly understood. Here, we perform measurements of transmon qubit relaxation times $T_1$ in parallel with spectroscopy and microscopy of the thin polycrystalline niobium films used in qubit fabrication. By comparing results for films deposited using three techniques, we reveal correlations between $T_1$ and grain size, enhanced oxygen diffusion along grain boundaries, and the concentration of suboxides near the surface. Physical mechanisms connect these microscopic properties to residual surface resistance and $T_1$ through losses arising from the grain boundaries and from defects in the suboxides. Further, experiments show that the residual resistance ratio can be used as a figure of merit for qubit lifetime. This comprehensive approach to understanding qubit decoherence charts a pathway for materials-driven improvements of superconducting qubit performance.",2004.02908v1 2021-01-23,Field-effect at electrical contacts to two-dimensional materials,"The inferior electrical contact to two-dimensional (2D) materials is a critical challenge for their application in post-silicon very large-scale integrated circuits. Electrical contacts were generally related to their resistive effect, quantified as contact resistance. With a systematic investigation, this work demonstrates a capacitive metal-insulator-semiconductor (MIS) field-effect at the electrical contacts to 2D materials: the field-effect depletes or accumulates charge carriers, redistributes the voltage potential, and give rise to abnormal current saturation and nonlinearity. On the one hand, the current saturation hinders the devices' driving ability, which can be eliminated with carefully engineered contact configurations. On the other hand, by introducing the nonlinearity to monolithic analog artificial neural network circuits, the circuits' perception ability can be significantly enhanced, as evidenced using a COVID-19 critical illness prediction model. This work provides a comprehension of the field-effect at the electrical contacts to 2D materials, which is fundamental to the design, simulation, and fabrication of electronics based on 2D material.",2101.09487v1 2022-05-30,Mechanistic framework for reduced-order models in soft materials: Application to three-dimensional granular intrusion,"Soft materials often display complex behaviors that transition through apparent solid- and fluid-like regimes. While a growing number of microscale simulation methods exist for these materials, reduced-order models that encapsulate the global-scale physics are often desired to predict how external bodies interact with soft media, as occurs in diverse situations from impact and penetration problems to locomotion over natural terrains. This work proposes a systematic program to develop three-dimensional reduced-order models for soft materials from a fundamental basis using continuum symmetries and rheological principles. In particular, we derive a reduced-order technique for modeling intrusion in granular media which we term three-dimensional Resistive Force Theory (3D-RFT), which is capable of accurately and quickly predicting the resistive stress distribution on arbitrary-shaped intruding bodies. Aided by a continuum description of the granular medium, a comprehensive set of spatial symmetry constraints, and a limited amount of reference data, we develop a self-consistent and accurate 3D-RFT. We verify the model capabilities in a wide range of cases and show it can be quickly recalibrated to different media and intruder surface types. The premises leading to 3D-RFT anticipate application to other soft materials with strongly hyperlocalized intrusion behavior.",2205.14920v3 2023-01-27,Machine-guided Design of Oxidation Resistant Superconductors for Quantum Information Applications,"Decoherence in superconducting qubits has long been attributed to two level systems arising from the surfaces and interfaces present in real devices. A recent significant step in reducing decoherence was the replacement of superconducting niobium by superconducting tantalum, resulting in a tripling of transmon qubit lifetimes (T1). One of these surface variables, the identity, thickness, and quality of the native surface oxide, is thought to play a major role as tantalum only has one oxide whereas niobium has several. Here we report the development of a thermodynamic metric to rank materials based on their potential to form a well-defined, thin, surface oxide. We first compute this metric for known binary and ternary metal alloys using data available from Materials Project, and experimentally validate the strengths and limits of this metric through preparation and controlled oxidation of 8 known metal alloys. Then we train a convolutional neural network to predict the value of this metric from atomic composition and atomic properties. This allows us to compute the metric for materials that are not present in materials project, including a large selection of known superconductors, and, when combined with Tc, allow us to identify new candidate superconductors for quantum information science (QISE) applications. We test the oxidation resistance of a pair of these predictions experimentally. Our results are expected to lay the foundation for tailored and rapid selection of improved superconductors for QISE.",2301.11543v1 2012-08-10,On the phase diagram of the itinerant helimagnet MnSi: does MnSi become quantum critical ?,"We performed a series of resistivity measurements of a MnSi single crystal at high pressures, created by a piston-cylinder device with a liquid pressure medium. The form of the resistivity curve at ambient pressure clearly indicates a first order nature of the magnetic phase transition in MnSi. Application of high pressure shows fast degradation of the first order features of the phase transition. The temperature derivative of resistivity demonstrates two notable features of the phase transition that disappear on pressure increasing. They are a sharp peak marking the first order phase transition and a shallow maximum, situated slightly above the critical temperature and pointing to the domain of prominent helical fluctuations. The current experimental data rule out any strong first order phase transition in MnSi at high pressures and low temperatures, which would prevent development of a quantum critical region. On the contrary, there should exist true quantum critical phenomena in MnSi at high pressures because a tiny first order transition, if it survives at high pressures to the lowest temperature, hardly could suppress the entire quantum critical region.",1208.2174v1 2017-04-12,High temperature resistivity measured at ν = 5/2 as a predictor of 2DEG quality in the N=1 Landau level,"We report a high temperature (T = 0.3K) indicator of the excitation gap $\Delta_{5/2}$ at the filling factor $ \nu=5/2$ fractional quantum Hall state in ultra-high quality AlGaAs/GaAs two-dimensional electron gases. As the lack of correlation between mobility $\mu$ and $\Delta_{5/2}$ has been well established in previous experiments, we define, analyze and discuss the utility of a different metric $\rho_{5/2}$, the resistivity at $\nu=5/2$, as a high temperature predictor of $\Delta_{5/2}$. This high-field resistivity reflects the scattering rate of composite fermions. Good correlation between $\rho_{5/2}$ and $\Delta_{5/2}$ is observed in both a density tunable device and in a series of identically structured wafers with similar density but vastly different mobility. This correlation can be explained by the fact that both $\rho_{5/2}$ and $\Delta_{5/2}$ are sensitive to long-range disorder from remote impurities, while $\mu$ is sensitive primarily to disorder localized near the quantum well.",1704.03794v1 2019-08-02,Realization of Ohmic-contact and velocity saturation in organic field-effect transistors by crystallized monolayer,"The contact resistance limits the down-scaling and operating range of OFETs. With the monolayer (1L) organic crystals and non-destructive metal/semiconductor interfaces, intrinsic mobility of 12.5 cm2V-1s-1 and Ohmic contact resistance of 40 ohm-cm were achieved. The on/off ratio maintained at 10^3 even at a small VDS of -0.1 mV. High current density of 4.2 uA/um was achieved with the 1L-crystal as the active layer. At such high current density, the velocity saturation and channel self-heating effects are observed in OFETs for the first time. In addition to the low contact resistance and high-resolution lithography, we suggest the thermal management of the high mobility OFETs will be the next major challenge to achieve high-speed densely integrated flexible electronics.",1908.01032v1 2022-11-04,Relativistic resistive magneto-hydrodynamics code for high-energy heavy-ion collisions,"We construct a relativistic resistive magneto-hydrodynamic (RRMHD) numerical simulation code for high-energy heavy-ion collisions. We split the system of differential equations into two parts, a non-stiff and a stiff part. For the non-stiff part, we evaluate the numerical flux using HLL approximated Riemann solver and execute the time integration by the second-order of Runge-Kutta algorithm. For the stiff part, which appears in Ampere's law, we integrate the equations using semi-analytic solutions of the electric field. We employ the generalized Lagrange multiplier method to ensure the divergence-free constraint for the magnetic field and Gauss's law. We confirm that our code reproduces well the results of standard RRMHD tests in the Cartesian coordinates. In the Milne coordinates, the code with high conductivity is validated against relativistic ideal MHD tests. We also verify the semi-analytic solutions of the accelerating longitudinal expansion of relativistic resistive magneto-hydrodynamics in high-energy heavy-ion collisions in a comparison with our numerical result. Our numerical code reproduces these solutions.",2211.02310v1 2022-02-28,Mg-doping and free-hole properties of hot-wall MOCVD GaN,"The hot-wall metal-organic chemical vapor deposition (MOCVD), previously shown to enable superior III-nitride material quality and high performance devices, has been explored for Mg doping of GaN. We have investigated the Mg incorporation in a wide doping range ($2.45\times{10}^{18}~cm^{-3}$ up to $1.10\times{10}^{20}~cm^{-3}$) and demonstrate GaN:Mg with low background impurity concentrations under optimized growth conditions. Dopant and impurity levels are discussed in view of Ga supersaturation which provides a unified concept to explain the complexity of growth conditions impact on Mg acceptor incorporation and compensation. The results are analysed in relation to the extended defects, revealed by scanning transmission electron microscopy (STEM), X-ray diffraction (XRD), and surface morphology, and in correlation with the electrical properties obtained by Hall effect and capacitance-voltage (C-V) measurements. This allows to establish a comprehensive picture of GaN:Mg growth by hot-wall MOCVD providing guidance for growth parameters optimization depending on the targeted application. We show that substantially lower H concentration as compared to Mg acceptors can be achieved in GaN:Mg without any in-situ or post-growth annealing resulting in p-type conductivity in as-grown material. State-of-the-art $p$-GaN layers with a low-resistivity and a high free-hole density (0.77 $\Omega$.cm and $8.4\times{10}^{17}~cm^{-3}$, respectively) are obtained after post-growth annealing demonstrating the viability of hot-wall MOCVD for growth of power electronic device structures.",2202.13614v1 2019-11-21,Oxidized-monolayer Tunneling Barrier for Strong Fermi-level Depinning in Layered InSe Transistors,"In 2D-semiconductor-based field-effect transistors and optoelectronic devices, metal-semiconductor junctions are one of the crucial factors determining device performance. The Fermi-level (FL) pinning effect, which commonly caused by interfacial gap states, severely limits the tunability of junction characteristics, including barrier height and contact resistance. A tunneling contact scheme has been suggested to address the FL pinning issue in metal-2D-semiconductor junctions, whereas the experimental realization is still elusive. Here, we show that an oxidized-monolayer-enabled tunneling barrier can realize a pronounced FL depinning in indium selenide (InSe) transistors, exhibiting a large pinning factor of 0.5 and a highly modulated Schottky barrier height. The FL depinning can be attributed to the suppression of metal- and disorder-induced gap states as a result of the high-quality tunneling contacts. Structural characterizations indicate uniform and atomically thin surface oxidation layer inherent from nature of van der Waals materials and atomically sharp oxide-2D-semiconductor interfaces. Moreover, by effectively lowering the Schottky barrier height, we achieve an electron mobility of 2160 cm$^2$/Vs and a contact barrier of 65 meV in two-terminal InSe transistors. The realization of strong FL depinning in high-mobility InSe transistors with the oxidized monolayer presents a viable strategy to exploit layered semiconductors in contact engineering for advanced electronics and optoelectronics.",1911.09327v1 2023-12-11,Development of travelling heater method for growth of detector grade CdZnTe single crystals,"We report on the indigenous design and development of laboratory scale travelling heater method (THM) system to grow detector grade Cd0.9Zn0.1Te (CdZnTe) single crystals. THM system mainly consists of two-zone furnace with a tuneable temperature gradient (30 - 80 C/cm), high precision translation (1 - 25 mm per day) and rotation (1 - 50 rpm) assemblies to meet the stringent conditions that are essential to grow detector grade CdZnTe single crystals. Further, a load cell in the THM system enables continuous monitoring of the growth. Systematic growth experiments were performed to optimize the various growth parameters in order to achieve large grain single crystals. Herein, the effect of temperature gradient and growth rate on the increase in grain size is discussed in detail. Each successful growth experiment yields a minimum of four detector grade elements of dimensions 10 x 10 x 5 mm3 from a starting charge of 100 g of CdZnTe. The crystalline nature and quality of the detector elements were evaluated using Laue, NIR transmission spectroscopy and I-V characteristics. Crystals with resistivity greater than ~ 1-10 giga-ohm-cm were identified for testing gamma ray detection. The photo peak of 137Cs was resolved with an energy resolution of 4.2 % at 662 keV and its measured electron mobility lifetime product is found to be ~ 3.3 x 10-3 cm2/V. The demonstration of the gamma ray detection with a relatively high {\mu}{\tau} product is the testimony to the successful growth of detector grade CdZnTe single crystals by an indigenously developed THM system.",2312.06233v1 2020-09-10,Water Within a Permanently Shadowed Lunar Crater: Further LCROSS Modeling and Analysis,"The 2009 Lunar CRater Observation and Sensing Satellite (LCROSS) impact mission detected water ice absorption using spectroscopic observations of the impact-generated debris plume taken by the Shepherding Spacecraft, confirming an existing hypothesis regarding the existence of water ice in permanently shadowed regions within Cabeus crater. Ground-based observations in support of the mission were able to further constrain the mass of the debris plume and the concentration of the water ice ejected during the impact. In this work, we explore additional constraints on the initial conditions of the pre-impact lunar sediment required in order to produce a plume model that is consistent with the ground-based observations. We match the observed debris plume lightcurve using a layer of dirty ice with an ice concentration that increases with depth, a layer of pure regolith, and a layer of material at about 6 meters below the lunar surface that would otherwise have been visible in the plume but has a high enough tensile strength to resist excavation. Among a few possible materials, a mixture of regolith and ice with a sufficiently high ice concentration could plausibly produce such a behavior. The vertical albedo profiles used in the best fit model allows us to calculate a pre-impact mass of water ice within Cabeus crater of $5 \pm 3.0 \times 10^{11}$ kg and a mass concentration of water in the lunar sediment of $8.2 \pm 0.001$ %wt, assuming a water ice albedo of 0.8 and a lunar regolith density of 1.5 g cm$^{-3}$, or a mass concentration of water of $4.3 \pm 0.01$ %wt, assuming a lunar regolith density of 3.0. These models fit to ground-based observations result in derived masses of regolith and water ice within the debris plume that are consistent with \emph{in situ} measurements, with a model debris plume ice mass of 108 kg.",2009.05080v1 2019-08-03,Real-time Deep Learning at the Edge for Scalable Reliability Modeling of Si-MOSFET Power Electronics Converters,"With the significant growth of advanced high-frequency power converters, on-line monitoring and active reliability assessment of power electronic devices are extremely crucial. This article presents a transformative approach, named Deep Learning Reliability Awareness of Converters at the Edge (Deep RACE), for real-time reliability modeling and prediction of high-frequency MOSFET power electronic converters. Deep RACE offers a holistic solution which comprises algorithm advances, and full system integration (from the cloud down to the edge node) to create a near real-time reliability awareness. On the algorithm side, this paper proposes a deep learning algorithmic solution based on stacked LSTM for collective reliability training and inference across collective MOSFET converters based on device resistance changes. Deep RACE also proposes an integrative edge-to-cloud solution to offer a scalable decentralized devices-specific reliability monitoring, awareness, and modeling. The MOSFET convertors are IoT devices which have been empowered with edge real-time deep learning processing capabilities. The proposed Deep RACE solution has been prototyped and implemented through learning from MOSFET data set provided by NASA. Our experimental results show an average miss prediction of $8.9\%$ over five different devices which is a much higher accuracy compared to well-known classical approaches (Kalman Filter, and Particle Filter). Deep RACE only requires $26ms$ processing time and $1.87W$ computing power on Edge IoT device.",1908.01244v1 2022-04-29,Quantitative Prediction of Fracture Toughness $(K_{{\rm I}c})$ of Polymer by Fractography Using Deep Neural Networks,"Fracture surfaces provide various types of information about fracture. The fracture toughness $K_{{\rm I}c}$, which represents the resistance to fracture, can be estimated using the three-dimensional (3D) information of a fracture surface, i.e., its roughness. However, this is time-consuming and expensive to obtain the 3D information of a fracture surface; thus, it is desirable to estimate $K_{{\rm I}c}$ from a two-dimensional (2D) image, which can be easily obtained. In recent years, methods of estimating a 3D structure from its 2D image using deep learning have been rapidly developed. In this study, we propose a framework for fractography that directly estimates $K_{{\rm I}c}$ from a 2D fracture surface image using deep neural networks (DNNs). Typically, image recognition using a DNN requires a tremendous amount of image data, which is difficult to acquire for fractography owing to the high experimental cost. To compensate for the limited data, in this study, we used the transfer learning (TL) method, and constructed high-performance prediction models even with a small dataset by transferring machine learning models trained using other large datasets. We found that the regression model obtained using our proposed framework can predict $K_{{\rm I}c}$ in the range of approximately 1-5 [MPa$\sqrt{m}$] with a standard deviation of the estimation error of approximately $\pm$0.37 [MPa$\sqrt{m}$]. The present results demonstrate that the DNN trained with TL opens a new route for quantitative fractography by which parameters of fracture process can be estimated from a fracture surface even with a small dataset. The proposed framework also enables the building of regression models in a few hours. Therefore, our framework enables us to screen a large number of image datasets available in the field of materials science and find candidates that are worth expensive machine learning analysis.",2204.13912v1 2023-06-26,Elucidating Interfacial Dynamics of Ti-Al Systems Using Molecular Dynamics Simulation and Markov State Modeling,"Due to their remarkable mechanical and chemical properties, Ti-Al based materials are attracting considerable interest in numerous fields of engineering, such as automotive, aerospace, and defense. With their low density, high strength, and resistance to corrosion and oxidation, these intermetallic alloys and compound metal-metallic composites have found diverse applications. The present study delves into the interfacial dynamics of these Ti-Al systems, particularly focusing on the behavior of Ti and Al atoms in the presence of TiAl$_3$ grain boundaries under experimental heat treatment conditions. Using a combination of Molecular Dynamics and Markov State Model analyses, we scrutinize the kinetic processes involved in the formation of TiAl$_3$. The Molecular Dynamics simulation indicates that at the early stage of heat treatment, the predominating process is the diffusion of Al atoms towards the Ti surface through the TiAl$_3$ grain boundaries. The Markov State Modeling identifies three distinct dynamic states of Al atoms within the Ti/Al mixture that forms during the process, each exhibiting a unique spatial distribution. Using transition timescales as a qualitative measure of the rapidness of the dynamics, it is observed that the Al dynamics is significantly less rapid near the Ti surface compared to the Al surface. Put together, the results offer a comprehensive understanding of the interfacial dynamics and reveals a three-stage diffusion mechanism. The process initiates with the premelting of Al, proceeds with the prevalent diffusion of Al atoms towards the Ti surface, and eventually ceases as the Ti concentration within the mixture progressively increases. The insights gained from this study could contribute significantly to the control and optimization of manufacturing processes for these high-performing Ti-Al based materials.",2306.14568v2 2024-01-17,Pressure-induced superconductivity in a novel germanium allotrope,"High-pressure studies on elements play an essential role in superconductivity research, with implications for both fundamental science and applications. Here we report the experimental discovery of surprisingly low pressure driving a novel germanium allotrope into a superconducting state in comparison to that for alpha-Ge. Raman measurements revealed structural phase transitions and possible electronic topological transitions under pressure up to 58 GPa. Based on pressure-dependent resistivity measurements, superconductivity was induced above 2 GPa and the maximum Tc of 6.8 K was observed under 4.6 GPa. Interestingly, a superconductivity enhancement was discovered during decompression, indicating the possibility of maintaining pressure-induced superconductivity at ambient pressure with better superconducting performance. Density functional theory analysis further suggested that the electronic structure of Ge (oP32) is sensitive to its detailed geometry and revealed that disorder in the beta-tin structure leads to a higher Tc in comparison to the perfect beta-tin Ge.",2401.09625v1 2012-01-09,Performances and ageing study of resistive-anodes Micromegas detectors for HL-LHC environment,"With the tenfold luminosity increase envisaged at the HL-LHC, the background (photons, neutrons, ...) and the event pile-up probability are expected to increase in proportion in the different experiments, especially in the forward regions like, for instance, the muons chambers of the ATLAS detector. Detectors based on the Micromegas principle should be good alternatives for the detector upgrade in the HL-LHC framework because of a good spatial (<100 \mum) and time (few ns) resolutions, high-rate capability, radiation hardness, good robustness and the possibility to build large areas. The aim of this study is to demonstrate that it is possible to reduce the discharge probability and protect the electronics by using a resistive anode plane in a high flux hadrons environment. Several prototypes of 10x10 cm2, with different pitches (0.5 to 2 mm) and different resistive layers have been tested at CERN (pi+@SPS). Several tests have been performed with a telescope at different voltages to assess the performances of the detectors in terms of position resolution and efficiency. The spark behaviour in these conditions has also been evaluated. Resistive coating has been shown to be a successful method to reduce the effect of sparks on the efficiency of micromegas. A good spatial resolution (~80 \mum) can be reached with a resistive strip coating detector of 1mm pitch and a high efficiency (> 98%) can be achieved with resistive-anode micromegas detector. An X-rays irradiation has been also performed, showing no ageing effect after more than 21 days exposure and an integrated charge of almost 1C.",1201.1843v1 2003-09-01,Non-equilibrium and non-linear stationary state in thermoelectric materials,"Efficiency of thermoelectric materials is characterized by the figure of merit Z. Z has been believed to be a peculiar material constant. However, the accurate measurements in the present work reveal that Z has large size dependence and a non-linear temperature distribution appears as stationary state in the thermoelectric material. The observation of these phenomena is achieved by the Harman method. This method is the most appropriate way to investigate the thermoelectric properties because the dc and ac resistances are measured by the same electrode configuration. We describe the anomalous thermoelectric properties observed in mainly (Bi,Sb)2Te3 by the Harman method and then insist that Z is not the peculiar material constant but must be defined as the physical quantity dependent of the size and the position in the material.",0309016v1 2006-11-27,Comparison of Methods for Characterizing Sound Absorbing Materials,"Sound absorbing materials are usually defined by five parameters: open porosity, static airflow resistivity, tortuosity, and two characteristic lengths. In recent decades, different methods have been developed in order to characterize these parameters. These methods may be divided following three approaches: i) inverse, ii) indirect and iii) direct. The inverse approach is based on an optimisation problem where the material parameters are adjusted in the acoustic model to reproduce acoustical measurements. The indirect approach is based on the acoustical model from which analytical expressions linking the material parameters to acoustical measurements are derived. Contrary to the previous two approaches, the direct approach is not based on acoustical measurements. It is based on the physical and mathematical definition of the parameters and requires dedicated equipments. In this study, the five parameters have been measured for different porous materials using some direct, indirect and inverse methods. A comparison of the different results is carried out, and shows that the different methods may yield large variability in the found parameters. A discussion is given to explain the observed variability and the limitations of the methods.",0611259v2 2007-08-14,Preliminary Results on Vibration Damping Properties of Nanoscale-Reinforced Composite Materials,"The focus in this paper is an analysis of existing state of the arts directed toward the development of the next generation of vibration damping systems. The research work concentrates on an investigation related to nanoparticles/fibres/tubes-reinforced materials and coatings dynamic characterization and modeling of the fundamental phenomena that control relationships between structure and damping/mechanical properties of the materials. We simulated composite materials using finite element and mesh free methods, using a hollow shell representation of the individual nanotube/fiber. Results of the research work will provide a platform for the development of nanoparticle-reinforced damping materials that are light-weight, vibration and shock resistant. The outcome of the research work is expected to have wide-ranging technical benefits with direct relevance to industry in areas of transportation (aerospace, automotive, rail), electronics and civil infrastructure development.",0708.1821v1 2018-05-25,Imaging material functionality through 3D nanoscale tracking of energy flow,"The ability of energy carriers to move between atoms and molecules underlies biochemical and material function. Understanding and controlling energy flow, however, requires observing it on ultrasmall and ultrafast spatiotemporal scales, where energetic and structural roadblocks dictate the fate of energy carriers. Here we developed a non-invasive optical scheme that leverages non-resonant interferometric scattering to track tiny changes in material polarizability created by energy carriers. We thus map evolving energy carrier distributions in four dimensions of spacetime with few-nanometer lateral precision and directly correlate to material morphology. We visualize exciton, charge, and heat transport in polyacene, silicon and perovskite semiconductors and elucidate how disorder affects energy flow in 3D. For example, we show that morphological boundaries in polycrystalline metal halide perovskites possess lateral- and depth-dependent resistivities, blocking lateral transport for surface but not bulk carriers. We furthermore reveal strategies to interpret energy transport in disordered environments that will direct the design of defect-tolerant materials for the semiconductor industry of tomorrow.",1805.09982v4 2020-03-30,A bioinspired optically transparent tough glass composite,"Glasses have numerous applications due to their exceptional transparency, however, poor fracture and impact resistance limit their applications as an engineering material. One relatively recent approach to improve the mechanical properties of materials is through bio-inspiration. Structural biological composites such as nacre, the protective inner layer of mollusk shells, offer far superior mechanical properties relative to their constituents. This has motivated researchers to mimic the design principles in natural composites to create tough transparent materials. However, current bio-inspired materials lack fabrication scalability or offer poor optical transmission. Here, an efficient, scalable bulk process is developed for creating optically transparent tough composites, resulting in a nacreous glass composite material with a four-fold increase in fracture toughness and a three-fold increase in flexural strength compared to conventional structural glasses, and with a 73% of average optical transmittance. The composite consists of glass flakes and poly (methyl methacrylate) (PMMA) assembled utilizing a centrifuge-based fabrication method that aligns and compacts the flakes into layers. To optimize the transparency of the structure, the refractive indices of the PMMA and glass are matched. Based on the results, this nacreous glass composite is proposed as a potential alternative in diverse architectural, vehicular, and electronics applications.",2003.13863v1 2021-04-15,Towards A Process Model for Co-Creating AI Experiences,"Thinking of technology as a design material is appealing. It encourages designers to explore the material's properties to understand its capabilities and limitations, a prerequisite to generative design thinking. However, as a material, AI resists this approach because its properties emerge as part of the design process itself. Therefore, designers and AI engineers must collaborate in new ways to create both the material and its application experience. We investigate the co-creation process through a design study with 10 pairs of designers and engineers. We find that design 'probes' with user data are a useful tool in defining AI materials. Through data probes, designers construct designerly representations of the envisioned AI experience (AIX) to identify desirable AI characteristics. Data probes facilitate divergent thinking, material testing, and design validation. Based on our findings, we propose a process model for co-creating AIX and offer design considerations for incorporating data probes in design tools.",2104.07595v2 2022-05-30,Progress and prospects in the quantum anomalous Hall effect,"The quantum anomalous Hall effect refers to the quantization of Hall effect in the absence of applied magnetic field. The quantum anomalous Hall effect is of topological nature and well suited for field-free resistance metrology and low-power information processing utilizing dissipationless chiral edge transport. In this Perspective, we provide an overview of the recent achievements as well as the materials challenges and opportunities, pertaining to engineering intrinsic/interfacial magnetic coupling, that are expected to propel future development of the field.",2205.15226v3 2023-07-09,lcs4Foam -- An OpenFOAM Function Object to Compute Lagrangian Coherent Structures,"To facilitate the understanding and to quantitatively assess the material transport in fluids, a modern characterisation method has emerged in fluid dynamics in the last decades footed in dynamical systems theory. It allows to examine the most influential material lines which are called Lagrangian Coherent Structures (LCS) and order the material transport into dynamically distinct regions at large scales which resist diffusion or mixing. LCS reveal the robust skeleton of material surfaces and are essential to assess material transport in time-dependent flows quantitatively. Candidates of LCS can be estimated and visualised from finite-time stretching and folding fields by calculating the Finite-Time Lyapunov Exponents (FTLE). In this contribution, we provide an OpenFOAM function object to compute FTLE during CFD simulation. This enables the OpenFOAM community to assess the geometry of the material transport in any flow quantitatively on-the-fly using principally any OpenFOAM flow solver.",2307.04104v1 2023-11-23,Rate- and temperature-dependent ductile-to-brittle fracture transition: Experimental investigation and phase-field analysis for toffee,"The mechanical behaviour of many materials, including polymers or natural materials, significantly depends on the rate of deformation. As a consequence, a rate-dependent ductile-to-brittle fracture transition may be observed. For toffee-like caramel, this effect is particularly pronounced. At room temperature, this confectionery may be extensively deformed at low strain rates, while it can behave highly brittle when the rate of deformation is raised. Likewise, the material behaviour does significantly depend on temperature, and even a slight cooling may cause a significant embrittlement. In this work, a thorough experimental investigation of the rate-dependent deformation and fracture behaviour is presented. In addition, the influence of temperature on the material response is studied. The experimental results form the basis for a phase-field modelling of fracture. In order to derive the governing equations of the model, an incremental variational principle is introduced. By means of the validated model, an analysis of the experimentally observed ductile-to-brittle fracture transition is performed. In particular, the coupling between the highly dissipative deformation behaviour of the bulk material and the rate-dependent fracture resistance is discussed.",2311.13869v1 2023-01-15,Inhomogeneous superconductivity onset in FeSe studied by transport properties,"Heterogeneous superconductivity onset is a common phenomenon in high-$T_c$ superconductors of both the cuprate and iron-based families. It is manifested by a fairly wide transition from the metallic to zero-resistance state. Usually, in these strongly anisotropic materials, superconductivity (SC) first appears as isolated domains. This leads to anisotropic excess conductivity above $T_c$, and the transport measurements provide valuable information about the SC domain structure deep within the sample. In bulk samples, this anisotropic SC onset gives an approximate average shape of SC grains, while in thin samples it also indicates the average size of SC grains. In this work, both interlayer and intralayer resistivity are measured as a function of temperature in FeSe samples of various thickness. To measure the interlayer resistivity, FeSe mesa structures oriented across the layers were fabricated using FIB. As the sample thickness decreases, a significant increase in superconducting transition temperature $T_c$ is observed : $T_c$ raises from 8 K in bulk material to 12 K in microbridges of thickness $\sim 40$ nm. We apply analytical and numerical calculations to analyze these and earlier data and find the aspect ratio and size of the SC domains in FeSe consistent with our resistivity and diamagnetic response measurements. We propose a simple and fairly accurate method for estimating the aspect ratio of SC domains from $T_c$ anisotropy in samples of various small thickness. The relationship between nematic and superconducting domains in FeSe is discussed. We also generalize the analytical formulas for conductivity in heterogeneous anisotropic superconductors to the case of elongated SC domains of two perpendicular orientations with equal volume fractions, corresponding to the nematic domain structure in various Fe-based superconductors.",2301.06185v3 2023-11-28,Sputtered NbN Films for Ultrahigh Performance Superconducting Nanowire Single-Photon Detectors,"Nowadays ultrahigh performance superconducting nanowire single-photon detectors are the key elements in a variety of devices from biological research to quantum communications and computing. Accurate tuning of superconducting material properties is a powerful resource for fabricating single-photon detectors with a desired properties. Here, we report on the major theoretical relations between ultrathin niobium nitride (NbN) films properties and superconducting nanowire single-photon detectors characteristics, as well as ultrathin NbN films properties dependence on reactive magnetron sputtering recipes. Based on this study we formulate the exact requirements to ultrathin NbN films for ultrahigh performance superconducting nanowire single-photon detectors. Then, we experimentally study ultrathin NbN films properties (morphology, crystalline structure, critical temperature, sheet resistance) on silicon, sapphire, silicon dioxide and silicon nitride substrates sputtered with various recipes. We demonstrate ultrathin NbN films (obtained with more than 100 films deposition) with a wide range of critical temperature from 2.5 to 12.1 K and sheet resistance from 285 to 2000 ~$\Omega$/sq, as well as investigate a sheet resistance evolution over for more than 40\% within two years. Finally, we found out that one should use ultrathin NbN films with specific critical temperature near 9 K and sheet resistance of 400 ~$\Omega$/sq for ultrahigh performance SNSPD.",2311.17000v1 2009-03-27,Very High Order $\PNM$ Schemes on Unstructured Meshes for the Resistive Relativistic MHD Equations,"In this paper we propose the first better than second order accurate method in space and time for the numerical solution of the resistive relativistic magnetohydrodynamics (RRMHD) equations on unstructured meshes in multiple space dimensions. The nonlinear system under consideration is purely hyperbolic and contains a source term, the one for the evolution of the electric field, that becomes stiff for low values of the resistivity. For the spatial discretization we propose to use high order $\PNM$ schemes as introduced in \cite{Dumbser2008} for hyperbolic conservation laws and a high order accurate unsplit time discretization is achieved using the element-local space-time discontinuous Galerkin approach proposed in \cite{DumbserEnauxToro} for one-dimensional balance laws with stiff source terms. The divergence free character of the magnetic field is accounted for through the divergence cleaning procedure of Dedner et al. \cite{Dedneretal}. To validate our high order method we first solve some numerical test cases for which exact analytical reference solutions are known and we also show numerical convergence studies in the stiff limit of the RRMHD equations using $\PNM$ schemes from third to fifth order of accuracy in space and time. We also present some applications with shock waves such as a classical shock tube problem with different values for the conductivity as well as a relativistic MHD rotor problem and the relativistic equivalent of the Orszag-Tang vortex problem. We have verified that the proposed method can handle equally well the resistive regime and the stiff limit of ideal relativistic MHD. For these reasons it provides a powerful tool for relativistic astrophysical simulations involving the appearance of magnetic reconnection.",0903.4832v1 2019-07-18,High-performance monolayer MoS2 field-effect transistor with large-scale nitrogen-doped graphene electrodes for Ohmic contact,"A finite Schottky barrier and large contact resistance between monolayer MoS2 and electrodes are the major bottlenecks in developing high-performance field-effect transistors (FETs) that hinder the study of intrinsic quantum behaviors such as valley-spin transport at low temperature. A gate-tunable graphene electrode platform has been developed to improve the performance of MoS2 FETs. However, intrinsic misalignment between the work function of pristine graphene and the conduction band of MoS2 results in a large threshold voltage for the FETs, because of which Ohmic contact behaviors are observed only at very high gate voltages and carrier concentrations (~1013 cm-2). Here, we present high-performance monolayer MoS2 FETs with Ohmic contact at a modest gate voltage by using a chemical-vapor-deposited (CVD) nitrogen-doped graphene with a high intrinsic electron carrier density. The CVD nitrogen-doped graphene and monolayer MoS2 hybrid FETs platform exhibited a large negative shifted threshold voltage of -54.2 V and barrier-free Ohmic contact under zero gate voltage. Transparent contact by nitrogen-doped graphene led to a 214% enhancement in the on-current and a four-fold improvement in the field-effect carrier mobility of monolayer MoS2 FETs compared with those of a pristine graphene electrode platform. The transport measurements, as well as Raman and X-ray photoelectron spectroscopy analyses before and after thermal annealing, reveal that the atomic C-N bonding in the CVD nitrogen-doped graphene is responsible for the dominant effects of electron doping. Large-scale nitrogen-doped graphene electrodes provide a promising device platform for the development of high-performance devices and the study of unique quantum behaviors.",1907.07883v1 2010-10-04,Defects induced ferromagnetism in Mn doped ZnO,"Single phase Mn doped (2 at %) ZnO samples have been synthesized by solid-state reaction technique. Before the final sintering at 500 C, the mixed powders have been milled for different milling periods (6, 24, 48 and 96 hours). The grain sizes of the samples are very close to each other (~ 32 \pm 4 nm). However, the defective state of the samples is different from each other as manifested from the variation of magnetic properties and electrical resistivity with milling time. All the samples have been found to be ferromagnetic with clear hysteresis loops at room temperature. The maximum value for saturation magnetization (0.11 {\mu}_B / Mn atom) was achieved for 96 hours milled sample. Electrical resistivity has been found to increase with increasing milling time. The most resistive sample bears the largest saturation magnetization. Variation of average positron lifetime with milling time bears a close similarity with that of the saturation magnetization. This indicates the key role played by open volume vacancy defects, presumably zinc vacancies near grain surfaces, in inducing ferromagnetic order in Mn doped ZnO. To attain optimum defect configuration favorable for ferromagnetism in this kind of samples proper choice of milling period and annealing conditions is required.",1010.0547v1 2013-04-11,Sign-reversal of the in-plane resistivity anisotropy in iron pnictides,"The concept of an electronically-driven breaking of the rotational symmetry of a crystal, without involving magnetic order, has found experimental support in several systems, from semiconductor heterostructures and ruthenates, to cuprate and iron-pnictide superconductors. In the pnictide BaFe$_{2}$As$_{2}$, such an ""electronic nematic state"" appears above the magnetic transition dome, over a temperature range that can be controlled by external strain. Here, by measuring the in-plane resistivity anisotropy, we probe the electronic anisotropy of this material over the entire nematic/magnetic dome, whose end points coincide with the optimal superconducting transition temperatures. Counter-intuitively, we find that, unlike other materials, the resistivity anisotropy in BaFe$_{2}$As$_{2}$ changes sign across the doping phase diagram, even though the signs of the magnetic, nematic, and orthorhombic order parameters are kept fixed. This behavior is explained by the Fermi surface reconstruction in the magnetic phase and spin-fluctuation scattering in the nematic phase. The unique behavior of the transport anisotropy unveils that the primary role is played by magnetic scattering in the normal state transport properties of the iron pnictides, suggesting a close connection between magnetism, nematicity, and unconventional superconductivity.",1304.3490v1 2013-09-20,Universal electric-field-driven resistive transition in narrow-gap Mott insulators,"One of today's most exciting research frontier and challenge in condensed matter physics is known as Mottronics, whose goal is to incorporate strong correlation effects into the realm of electronics. In fact, taming the Mott insulator-to-metal transition (IMT), which is driven by strong electronic correlation effects, holds the promise of a commutation speed set by a quantum transition, and with negligible power dissipation. In this context, one possible route to control the Mott transition is to electrostatically dope the systems using strong dielectrics, in FET-like devices. Another possibility is through resistive switching, that is, to induce the insulator-to-metal transition by strong electric pulsing. This action brings the correlated system far from equilibrium, rendering the exact treatment of the problem a difficult challenge. Here, we show that existing theoretical predictions of the off-equilibrium manybody problem err by orders of magnitudes, when compared to experiments that we performed on three prototypical narrow gap Mott systems V2-xCrxO3, NiS2-xSex and GaTa4Se8, and which also demonstrate a striking universality of this Mott resistive transition (MRT). We then introduce and numerically study a model based on key theoretically known physical features of the Mott phenomenon in the Hubbard model. We find that our model predictions are in very good agreement with the observed universal MRT and with a non-trivial timedelay electric pulsing experiment, which we also report. Our study demonstrates that the MRT can be associated to a dynamically directed avalanche.",1309.5315v1 2016-04-23,"Giant magnetoresistance, three-dimensional Fermi surface and origin of resistivity plateau in YSb semimetal","Very strong magnetoresistance and a resistivity plateau impeding low temperature divergence due to insulating bulk are hallmarks of topological insulators and are also present in topological semimetals where the plateau is induced by magnetic field, when time-reversal symmetry (protecting surface states in topological insulators) is broken. Similar features were observed in a simple rock-salt-structure LaSb, leading to a suggestion of the possible non-trivial topology of 2D states in this compound. We show that its sister compound YSb is also characterized by giant magnetoresistance exceeding one thousand percent and low-temperature plateau of resistivity. We thus performed in-depth analysis of YSb Fermi surface by band calculations, magnetoresistance, and Shubnikov--de Haas effect measurements, which reveals only three-dimensional Fermi sheets. Kohler scaling applied to magnetoresistance data accounts very well for its low-temperature upturn behavior. The field-angle-dependent magnetoresistance demonstrates a 3D-scaling yielding effective mass anisotropy perfectly agreeing with electronic structure and quantum oscillations analysis, thus providing further support for 3D-Fermi surface scenario of magnetotransport, without necessity of invoking topologically non-trivial 2D states. We discuss data implying that analogous field-induced properties of LaSb can also be well understood in the framework of 3D multiband model.",1604.06945v3 2017-02-23,Metallicity without quasi-particles in room-temperature strontium titanate,"Cooling oxygen-deficient strontium titanate to liquid-helium temperature leads to a decrease in its electrical resistivity by several orders of magnitude. The temperature dependence of resistivity follows a rough T$^{3}$ behavior before becoming T$^{2}$ in the low-temperature limit, as expected in a Fermi liquid. Here, we show that the roughly cubic resistivity above 100K corresponds to a regime where the quasi-particle mean-free-path is shorter than the electron wave-length and the interatomic distance. These criteria define the Mott-Ioffe-Regel limit. Exceeding this limit is the hallmark of strange metallicity, which occurs in strontium titanate well below room temperature, in contrast to other perovskytes. We argue that the T$^{3}$-resistivity cannot be accounted for by electron-phonon scattering \`{a} la Bloch-Gruneisen and consider an alternative scheme based on Landauer transmission between individual dopants hosting large polarons. We find a scaling relationship between the carrier mobility, the electric permittivity and the frequency of transverse optical soft mode in this temperature range. Providing an account of this observation emerges as a challenge to theory.",1702.07144v3 2018-02-26,Thermoelectric signatures of the electron-phonon fluid in PtSn4,"In most materials, transport can be described by the motion of distinct species of quasiparticles, such as electrons and phonons. Strong interactions between quasiparticles, however, can lead to collective behaviour, including the possibility of viscous hydrodynamic flow. In the case of electrons and phonons, an electron-phonon fluid is expected to exhibit strong phonon-drag transport signatures and an anomalously low thermal conductivity. The Dirac semi-metal PtSn4 has a very low resistivity at low temperatures and shows a pronounced phonon drag peak in the low temperature thermopower; it is therefore an excellent candidate for hosting a hydrodynamic electron-phonon fluid. Here we report measurements of the temperature and magnetic field dependence of the longitudinal and Hall electrical resistivities, the thermopower and the thermal conductivity of PtSn4. We confirm a phonon drag peak in the thermopower near 14 K and observe a concurrent breakdown of the Lorenz ratio below the Sommerfeld value. Both of these facts are expected for an electron-phonon fluid with a quasi-conserved total momentum. A hierarchy between momentum-conserving and momentum-relaxing scattering timescales is corroborated through measurements of the magnetic field dependence of the electrical and Hall resistivity and of the thermal conductivity. These results show that PtSn4 exhibits key features of hydrodynamic transport.",1802.09468v1 2018-11-23,Neuromorphic MoS2 memtransistors fabricated by localised helium ion beam irradiation,"Two-dimensional layered semiconductors have recently emerged as attractive building blocks for next-generation low-power non-volatile memories. However, challenges remain in the controllable sub-micron fabrication of bipolar resistively switching circuit components from these novel materials. Here we report on the scalable experimental realisation of lateral on-dielectric memtransistors from monolayer single-crystal molybdenum disulfide (MoS2) utilising a focused helium ion beam. Site-specific irradiation with the probe of a helium ion microscope (HIM) allows for the creation of charged defects in the MoS2 lattice. The reversible drift of these locally seeded defects in the applied electric field modulates the resistance of the semiconducting channel, enabling versatile memristive functionality on the nanoscale. We find the device can reliably retain its resistance ratios and set biases for hundreds of switching cycles at sweep frequencies of up to 2.9 V/s with relatively low drain-source biases. We also demonstrate long-term potentiation and depression with sharp habituation that promises application in future neuromorphic architectures. This work advances the down-scaling progress of memristive devices without sacrificing key performance parameters such as power consumption or its applicability for synaptic emulation.",1811.09545v1 2019-02-23,Quasi-ballistic thermal transport across MoS$_2$ thin films,"Layered two-dimensional (2D) materials have highly anisotropic thermal properties between the in-plane and cross-plane directions. In general, it is thought that cross-plane thermal conductivities ($\kappa_z$) are low, and therefore c-axis phonon mean free paths (MFPs) are small. Here, we measure $\kappa_z$ across MoS$_2$ films of varying thickness (20 to 240 nm) and uncover evidence of very long c-axis phonon MFPs at room temperature in these layered semiconductors. Experimental data obtained using time-domain thermoreflectance (TDTR) are in good agreement with first-principles density functional theory (DFT). These calculations reveal that ~50% of the heat is carried by phonons with MFP >200 nm, exceeding kinetic theory estimates by nearly two orders of magnitude. Because of quasi-ballistic effects, the $\kappa_z$ of nanometer thin films of MoS$_2$ scales with their thickness and the volumetric thermal resistance asymptotes to a non-zero value, ~10 m$^{2}$KGW$^{-1}$. This contributes as much as 30% to the total thermal resistance of a 20 nm thick film, the rest being limited by thermal interface resistance with the SiO$_2$ substrate and top-side aluminum transducer. These findings are essential for understanding heat flow across nanometer-thin films of MoS$_2$ for optoelectronic and thermoelectric applications.",1902.08713v2 2016-03-16,Coexistence of topological Dirac fermions in the surface and three-dimensional Dirac cone state in the bulk of ZrTe$_{5}$ single crystal,"Although, the long-standing debate on the resistivity anomaly in ZrTe$_{5}$ somewhat comes to an end, the exact topological nature of the electronic band structure remains elusive till today. Theoretical calculations predicted that bulk ZrTe$_{5}$ to be either a weak or a strong three-dimensional (3D) topological insulator. However, the angle resolved photoemission spectroscopy and transport measurements clearly demonstrate 3D Dirac cone state with a small mass gap between the valence band and conduction band in the bulk. From the magnetization and magneto-transport measurements on ZrTe$_{5}$ single crystal, we have detected both the signature of helical spin texture from topological surface state and chiral anomaly associated with the 3D Dirac cone state in the bulk. This implies that ZrTe$_{5}$ is a novel 3D topological insulator having massless Dirac fermionic excitation in its bulk gap state. Whereas, no 3D topological insulator known in material science holds linear band dispersion in its insulating bulk. Apart from the band topology, it is also apparent from the resistivity and Hall measurements that the anomalous peak in the resistivity can be shifted to a much lower temperature ($T$$<$2 K) by controlling impurity and defects.",1603.05175v2 2018-12-03,Effect of structure and composition on the electronic excitation induced amorphization of La$_2$Ti$_{2-x}$Zr$_x$O$_7$ ceramics,"Understanding the response of ceramics operating in extreme environments is of interest for a variety of applications. Ab initio molecular dynamic simulations have been used to investigate the effect of structure and $B$-site (=Ti, Zr) cation composition of lanthanum-based oxides (La$_2$$B_2$O$_7$) on electronic-excitation-induced amorphization. We find that the amorphous transition in monoclinic layered perovskite La$_2$Ti$_2$O$_7$ occurs for a lower degree of electronic excitation than for cubic pyrochlore La$_2$Zr$_2$O$_7$. While in each case the formation of O$_2$-like molecules drives the structure to an amorphous state, an analysis of the polyhedral connection network reveals that the rotation of TiO$_6$ octahedra in the monoclinic phase can promote such molecule formation, while such octahedral rotation is not possible in the cubic phase. However, once the symmetry of the cubic structure is broken by substituting Ti for Zr, it becomes less resistant to amorphization. A compound made of 50% Ti and 50% Zr (La$_2$TiZrO$_7$) is found to be more resistant in the monoclinic than in the cubic phase, which may be related to the lower bandgap of the cubic phase. These results illustrate the complex interplay of structure and composition that give rise to the radiation resistance of these important functional materials.",1812.01136v1 2019-11-09,Pulsed laser deposition of single phase n- and p-type Cu2O thin films with low resistivity,"Low resistivity (~3-24 mOhm.cm) with tunable n- and p-type phase pure Cu2O thin films have been grown by pulsed laser deposition at 25-200 0C by varying the background oxygen partial pressure (O2pp). Capacitance data obtained by electrochemical impedance spectroscopy was used to determine the conductivity (n- or p-type), carrier density, and flat band potentials for samples grown on indium tin oxide (ITO) at 25 0C. The Hall mobility of the n- and p-type Cu2O was estimated to be ~ 0.85 cm2.V-1s-1 and ~ 4.78 cm2.V-1s-1 respectively for samples grown on quartz substrate at 25 0C. An elevated substrate temperature ~ 200 0C with O2pp = 2 - 3 mTorr yielded p-type Cu2O films with six orders of magnitude higher resistivities in the range ~ 9 - 49 kOhm.cm and mobilities in the range ~ 13.5 - 22.2 cm2.V-1s-1. UV-Vis-NIR diffuse reflectance spectroscopy showed optical bandgaps of Cu2O films in the range of 1.76 to 2.15 eV depending on O2pp. Thin films grown at oxygen-rich conditions O2pp > 7 mTorr yielded mixed-phase copper oxide irrespective of the substrate temperatures and upon air annealing at 550 0C for 1 hour completely converted to CuO phase with n-type semiconducting properties (~12 Ohm.cm, ~1.50 cm2.V-1s-1). The as-grown p- and n-type Cu2O showed rectification and a photovoltaic (PV) response in solid junctions with n-ZnO and p-Si electrodes respectively. Our findings may create new opportunities for devising Cu2O based junctions requiring low process temperatures.",1911.03727v2 2019-11-13,Light Intensity Modulated Impedance Spectroscopy (LIMIS) in All-Solid-State Solar Cells at Open Circuit,"Potentiostatic impedance spectroscopy (IS) is a well stablished characterization technique for elucidating the electric resistivity and capacitive features of materials and devices. In the case of solar cells, by applying a small voltage perturbation the current signal is recorded and the recombination processes and defect distributions are among the typical outcomes in IS studies. In this work a photo-impedance approach, named light intensity modulated impedance spectroscopy (LIMIS), is first tested in all-solid-state photovoltaic cells by recording the individual photocurrent (IMPS) and photovoltage (IMVS) responsivity signals due to a small light perturbation at open-circuit (OC), and combining them: LIMIS=IMVS/IMPS. The experimental LIMIS spectra from silicon, organic, and perovskite solar cells are presented and compared with IS. An analysis of the equivalent circuit numerical models for total resistive and capacitive features is discussed. Our theoretical findings show a correction to the lifetimes evaluations by obtaining the total differential resistances and capacitances combining IS and LIMIS measurements. This correction addresses the discrepancies among different techniques, as shown with transient photovoltage. The experimental differences between IS and LIMIS (i) proves the unviability of the superposition principle, (ii) suggest a bias-dependent photo-current correction to the empirical Shockley equation of the steady-state current at different illumination intensities around OC and (iii) are proposed as a potential figure of merit for characterizing performance and stability of solar cells. In addition, new features are reported for the low-frequency capacitance of perovskite solar cells, measured by IS and LIMIS.",1911.05440v1 2020-01-19,Multilevel Resistance Switching and Enhanced Spin Transition Temperature in Single Molecule Spin Crossover Nanogap Devices,"Spin crossover (SCO) molecules are promising bi-stable magnetic switches with applications in molecular spintronics. However, little is known about the switching effects of a single SCO molecule when it is confined between two metal electrodes. Here we examine the switching properties of a [Fe(III)(EtOSalPet )(NCS)] SCO molecule that is specifically tailored for surface deposition and binding to only one gold electrode in a nanogap device. Temperature dependent conductivity measurements on SCO molecule containing electromigrated gold break junctions show voltage independent telegraphic-like switching between two resistance states at temperature below 200 K. The transition temperature is very different from the transition temperature of 83 K that occurs in a bulk film of the same material. This indicates that the bulk, co-operative SCO phenomenon is no longer preserved for a single molecule and that the surface interaction drastically increases the temperature of the SCO phenomenon. Another key finding of this work is that some devices show switching between multiple resistance levels. We propose that in this case, two SCO molecules are present within the nanogap with both participating in the electronic transport and switching.",2001.06879v1 2020-05-18,Muiltiscale modeling of electrical conductivity of R-BAPB polyimide + carbon nanotubes nanocomposites,"The electrical conductivity of the polyimide R-BAPB polymer filled with single-wall carbon nanotubes (CNT) with chirality (5,5) is modeled using a multi-scale approach. The modeling starts with molecular dynamics simulations of time-dependent fluctuating atomic configurations of polymer filled CNTs junctions. Then the atomic positions obtained in the first step are used to perform fully first-principles microscopic calculations of the CNTs junctions contact resistances using the Green's function based quantum transport technique. And finally, those contact resistances are supplied as an input to a statistical calculation of a CNTs ensemble conductivity using a Monte Carlo percolation model. The results of the first-principles calculations show a very strong dependence of the polymer filled CNTs junctions contact resistance on the geometry of CNTs junctions, including an angle $\varphi$ between nanotubes axes and the positions of polymer atoms around CNTs. Incorporating into the percolation model this strong dependence as well as CNTs agglomeration, pushed the calculated values of electrical conductivity just above the percolation threshold below 0.01 S/m, which is within the experimental range for composites with various base polymers. Possible mechanisms for further reduction of composites conductivity are discussed.",2005.09115v1 2020-07-09,Large magnetoresistance and non-zero Berry phase in the nodal-line semimetal MoO2,"We performed calculations of the electronic band structure and the Fermi surface as well as measured the longitudinal resistivity rhoxx(T,H), Hall resistivity rhoxy(T,H) and quantum oscillations of the magnetization as a function of temperature at various magnetic fields for MoO2 with monoclinic crystal structure. The band structure calculations show that MoO2 is a nodal-line semimetal when spin-orbit coupling is ignored. It was found that a large magnetoresistance reaching 5.03x10^4% at 2 K and 9 T, its nearly quadratic field dependence and a field-induced up-turn behavior of rhoxx(T), the characteristics common for many topologically non-trivial as well as trivial semimetals, emerge also in MoO2. The observed properties are attributed to a perfect charge-carrier compensation, evidenced by both calculations relying on the Fermi surface topology and the Hall resistivity measurements. Both the observation of negative magnetoresistance for magnetic field along the current direction and the non-zero Berry phase in de Haas-van Alphen measurements indicate that pairs of Weyl points appear in MoO2, which may be due to the crystal symmetry breaking. These results highlight MoO2 as a new platform materials for studying the topological properties of oxides.",2007.04814v1 2020-08-20,Origin of the hump anomalies in the Hall resistance loops of ultrathin SrRuO$_3$/SrIrO$_3$ multilayers,"The proposal that very small N\'eel skyrmions can form in SrRuO$_3$/SrIrO$_3$ epitaxial bilayers and that the electric field-effect can be used to manipulate these skyrmions in gated devices strongly stimulated the recent research of SrRuO$_3$ heterostructures. A strong interfacial Dzyaloshinskii-Moriya interaction, combined with the breaking of inversion symmetry, was considered as the driving force for the formation of skyrmions in SrRuO$_3$/SrIrO$_3$ bilayers. Here, we investigated nominally symmetric heterostructures in which an ultrathin ferromagnetic SrRuO$_3$ layer is sandwiched between large spin-orbit coupling SrIrO$_3$ layers, for which the conditions are not favorable for the emergence of a net interfacial Dzyaloshinskii-Moriya interaction. Previously the formation of skyrmions in the asymmetric SrRuO$_3$/SrIrO$_3$ bilayers was inferred from anomalous Hall resistance loops showing humplike features that resembled topological Hall effect contributions. Symmetric SrIrO$_3$/SrRuO$_3$/SrIrO$_3$ trilayers do not show hump anomalies in the Hall loops. However, the anomalous Hall resistance loops of symmetric multilayers, in which the trilayer is stacked several times, do exhibit the humplike structures, similar to the asymmetric SrRuO$_3$/SrIrO$_3$ bilayers. The origin of the Hall effect loop anomalies likely resides in unavoidable differences in the electronic and magnetic properties of the individual SrRuO$_3$ layers rather than in the formation of skyrmions.",2008.09028v3 2021-09-28,Transport anomalies in the layered compound BaPt4Se6,"We report a layered ternary selenide BaPt4Se6 featuring sesqui-selenide Pt2Se3 layers sandwiched by Ba atoms. The Pt2Se3 layers in this compound can be derived from the Dirac-semimetal PtSe2 phase with Se vacancies that form a honeycomb structure. This structure results in a Pt (VI) and Pt (II) mixed-valence compound with both PtSe6 octahedra and PtSe4 square net coordination configurations. Temperature dependent electrical transport measurements suggest two distinct anomalies: a resistivity crossover, mimic to the metal-insulator (M-I) transition at ~150K, and a resistivity plateau at temperatures below 10K. The resistivity crossover is not associated with any structural, magnetic or charge order modulated phase transitions. Magnetoresistivity, Hall and heat capacity measurements concurrently suggest an existing hidden state below 5K in this system. Angle-resolved photoemission spectroscopy measurements reveal a metallic state and no dramatic reconstruction of the electronic structure up to 200K.",2109.13902v1 2022-05-26,Is the optical conductivity of heavy fermion strange metals Planckian?,"Strange metal behavior appears across a variety of condensed matter settings and beyond, and achieving a universal understanding is an exciting prospect. The beyond-Landau quantum criticality of Kondo destruction has had considerable success in describing the behavior of strange metal heavy fermion compounds, and there is some evidence that the associated partial localization-delocalization nature can be generalized to diverse materials classes. Other potential overarching principles at play are also being explored. An intriguing proposal is that Planckian scattering, with a rate of $k_{\rm B}T/\hbar$, leads to the linear temperature dependence of the (dc) electrical resistivity, which is a hallmark of strange metal behavior. Here we extend a previously introduced analysis scheme based on the Drude description of the dc resistivity to optical conductivity data. When they are well described by a simple (ac) Drude model, the scattering rate can be directly extracted. This avoids the need to determine the ratio of charge carrier concentration to effective mass, which has complicated previous analyses based on the dc resistivity. However, we point out that strange metals typically exhibit strong deviations from Drude behavior, as exemplified by the ``extreme'' strange metal YbRh$_2$Si$_2$. This calls for alternative approaches, and we point to the power of strange metal dynamical (energy-over-temperature) scaling analyses for the inelastic part of the optical conductivity. If such scaling extends to the low-frequency limit, a strange metal relaxation rate can be estimated, and may ultimately be used to test whether strange metals relax in a Planckian manner.",2205.13382v2 2023-01-01,Characteristic lengthscales of the electrically-induced insulator-to-metal transition,"Some correlated materials display an insulator-to-metal transition as the temperature is increased. In most cases this transition can also be induced electrically, resulting in volatile resistive switching due to the formation of a conducting filament. While this phenomenon has attracted much attention due to potential applications, many fundamental questions remain unaddressed. One of them is its characteristic lengths: what sets the size of these filaments, and how does this impact resistive switching properties. Here we use a combination of wide-field and scattering-type scanning near-field optical microscopies to characterize filament formation in NdNiO3 and SmNiO3 thin films. We find a clear trend: smaller filaments increase the current density, yielding sharper switching and a larger resistive drop. With the aid of numerical simulations, we discuss the parameters controlling the filament width and, hence, the switching properties.",2301.00456v1 2023-03-01,Piezoelectric composite cements: Towards the development of self-powered and self-diagnostic materials,"Piezoresistivity is the most commonly used sensing principle in cement-based smart composites for strain-monitoring applications. Nonetheless, the need for external electric power to conduct electrical resistivity measurements restricts the scalability of this technology, especially when implemented in remote structures. To address this issue, this manuscript thoroughly analyzes the piezoelectric properties of cement composites doped with reduced graphene oxide (rGO) and evaluates their potential as self-powered strain sensors. To do so, a comprehensive methodology involving voltammetry measurements, open circuit potential determination, and uniaxial compression testing is developed to determine the piezoelectric coefficients of charge $d_{33}$ and voltage $g_{33}$. Furthermore, a novel circuital model for signal processing of the electromechanical response is developed and experimentally validated in terms of time series of output voltage, resistance, and the generated electric power. The developed methodology is applied to laboratory samples manufactured following two different filler dispersion methods. The presented results evidence that samples prepared by ultrasonic cleaner dispersion achieve optimal properties, with a piezoelectric charge coefficient of 1122.28$\mathrm{\pm}$246.67 pC/N, about 47 times greater than previously reported composites in the literature. Unlike piezoresistive cement-based composites, a remarkable nonlinear correlation between the fractional change in the intrinsic resistance of the material and the applied mechanical strain has been observed. Instead, a considerable linearity ($\mathrm{R^2}=0.96$) between the externally applied mechanical strain and the generated (piezoelectric) electric power has been found, which suggests the great potential of the latter for conducting off-the-grid strain monitoring applications.",2303.00352v1 2023-09-13,Anomalous Hall effect and magnetoresistance in micro-ribbons of the magnetic Weyl semimetal candidate PrRhC2,"PrRhC2 belongs to the rare-earth carbides family whose properties are of special interest among topological semimetals due to the simultaneous breaking of both inversion and time-reversal symmetry. The concomitant absence of both symmetries grants the possibility to tune the Weyl nodes chirality and to enhance topological effects like the chiral anomaly. In this work, we report on the synthesis and compare the magnetotransport measurements of a poly- and single crystalline PrRhC2 sample. Using a remarkable and sophisticated technique, the PrRhC2 single crystal is prepared via focused ion beam cutting from the polycrystalline material. Our magnetometric and specific heat analyses reveal a non-collinear antiferromagnetic state below 20K, as well as short-range magnetic correlations and/or magnetic fluctuations well above the onset of the magnetic transition. The transport measurements on the PrRhC2 single crystal display an electrical resistivity peak at 3K and an anomalous Hall effect below 6K indicative of a net magnetization component in the ordered state. Furthermore, we study the angular variation of magnetoresistivities as a function of the angle between the in-plane magnetic field and the injected electrical current. We find that both the transverse and the longitudinal resistivities exhibit fourfold angular dependencies due to higher-order terms in the resistivity tensor, consistent with the orthorhombic crystal symmetry of PrRhC2. Our experimental results may be interpreted as features of topological Weyl semimetallic behavior in the magnetotransport properties.",2309.06963v1 2024-03-25,"Electrically tunable, rapid spin-orbit torque induced modulation of colossal magnetoresistance in Mn$_3$Si$_2$Te$_6$ nanoflakes","As a quasi-layered ferrimagnetic material, Mn$_3$Si$_2$Te$_6$ nanoflakes exhibit magnetoresistance behaviour that is fundamentally different from their bulk crystal counterparts. They offer three key properties crucial for spintronics. Firstly, at least 10^6 times faster response comparing to that exhibited by bulk crystals has been observed in current-controlled resistance and magnetoresistance. Secondly, ultra-low current density is required for resistance modulation (~ 5 A/cm$^2$). Thirdly, electrically gate-tunable magnetoresistance has been realized. Theoretical calculations reveal that the unique magnetoresistance behaviour in the Mn$_3$Si$_2$Te$_6$ nanoflakes arises from a magnetic field induced band gap shift across the Fermi level. The rapid current induced resistance variation is attributed to spin-orbit torque, an intrinsically ultra-fast process (~nanoseconds). This study suggests promising avenues for spintronic applications. In addition, it highlights Mn$_3$Si$_2$Te$_6$ nanoflakes as a suitable platform for investigating the intriguing physics underlying chiral orbital moments, magnetic field induced band variation and spin torque.",2403.16684v1 2004-09-16,Oscillatory and Vanishing Resistance States in Microwave Irradiated 2D Electron Systems,"Giant-amplitude oscillations in dc magnetoresistance of a high-mobility two-dimensional electron system can be induced by millimeterwave irradiations, leading to zero-resistance states at the oscillation minima. Following a brief overview of the now well-known phenomenon, this paper reports on aspects of more recent experiments on the subject. These are: new zero-resistance states associated with multi-photon processes; suppression of Shubnikov-de Haas oscillations by high-frequency microwaves; and microwave photoconductivity of a high-mobility two-dimensional hole system.",0409409v2 2010-02-09,Pressure-induced high-Tc superconducting phase in FeSe: correlation between anion height and Tc,"In this study, we performed high-pressure electrical resistivity measurements of polycrystalline FeSe in the pressure range of 1-16.0 GPa at temperatures of 4-300 K. A precise evaluation of Tc from zero-resistivity temperatures revealed that Tc shows a slightly distorted dome-shaped curve, with maximum Tc (30 K) at 6 GPa, which is lower than a previously reported Tc value (~37 K). With the application of pressure, the temperature dependence of resistivity above Tc changes dramatically to a linear dependence; a non-Fermi-liquid-like ""high-Tc"" phase appears above 3 GPa. We found a striking correlation between Tc and the Se height: the lower the Se height, the more enhanced is Tc. Moreover, this relation is broadly applicable to other iron pnictides, strongly indicating that high-temperature superconductivity can appear only around the optimum anion height (~1.38A). On the basis of these results, we suggest that the anion height should be considered as a key determining factor of Tc of iron-based superconductors containing various anions.",1002.1832v2 2017-06-22,Magneto-resistance oscillations induced by high-intensity terahertz radiation,"We report on observation of pronounced terahertz radiation-induced magneto-resistivity oscillations in AlGaAs/GaAs two-dimensional electron systems, the THz analog of the microwave induced resistivity oscillations (MIRO). Applying high power radiation of a pulsed molecular laser we demonstrate that MIRO, so far observed at low power only, are not destroyed even at very high intensities. Experiments with radiation intensity ranging over five orders of magnitude from $0.1$ W/cm$^2$ to $10^4$ W/cm$^2$ reveal high-power saturation of the MIRO amplitude, which is well described by an empirical fit function $I/(1 + I/I_s)^\beta$ with $\beta \sim 1$. The saturation intensity Is is of the order of tens of W/cm$^2$ and increases by six times by increasing the radiation frequency from $0.6$ to $1.1$ THz. The results are discussed in terms of microscopic mechanisms of MIRO and compared to nonlinear effects observed earlier at significantly lower excitation frequencies.",1706.07239v1 2019-08-10,High-resistance YBa2Cu3O7-x grain-boundary Josephson junctions fabricated by electromigration,"[100]-tilt grain-boundary YBa2Cu3O7-x (YBCO) junctions are promising for investigation of macroscopic quantum phenomena in high-Tc Josephson junctions. However, fabrication of the [100]-tilt grain-boundary YBCO junctions with a high resistance, which are required to study quantum effects, is difficult because of a high transparency of a tunnel barrier in this type of junctions. Here, we demonstrate a modification of grain-boundary barrier properties with a new approach to an oxygen electromigration in the YBCO grain-boundary junctions when the oxygen diffuses under an applied electric field from the grain-boundary to a BaTbO3 layer deposited atop of an YBCO film. Using this approach, we changed the normal-state resistance of the junctions from tens to several hundred Ohms without a degradation of their characteristic voltage IcRn and determined a barrier height and thickness by measuring the quasiparticle tunnelling current.",1908.03784v1 1995-01-26,Study of the band--gap shift in CdS films: Influence of thermal annealing in different atmospheres,"We study by photoacoustic spectroscopy the band--gap shift effect of CdS films. The CdS films were grown by chemical bath deposition and exposed to different annealing atmospheres over a range of temperature in which the sample structure is observed to change. We show the band--gap evolution as a function of temperature of thermal annealing and determine the process which produces the best combination of high band--gap energy and low resistivity. It allows us to know a possible procedure to obtain low--resistivity CdS/CdTe solar cells with high--quantum efficiency.",9501125v1 1995-07-14,Spin Conductivity and Spin-Charge Separation in the High $T_c$ Cuprates,"We study both the spin and electrical conductivities in models of relevance to the high $T_c$ cuprates. These models describe metallic states with or without spin-charge separation. We demonstrate that, given a linear in temperature dependence of the electrical resistivity, the spin resistivity should also be linear in temperature in the absence of spin-charge separation and under conditions appropriate at least for the optimally doped cuprates, but is in general {\it not} so in the presence of spin-charge separation. Based on these results, we propose to use the temperature dependence of the electron spin diffusion constant to diagnose spin-charge separation in the cuprates.",9507050v1 1997-08-15,Metal Insulator transition at B=0 in p-SiGe,"Observations are reported of a metal-insulator transition in a 2D hole gas in asymmetrically doped strained SiGe quantum wells. The metallic phase, which appears at low temperatures in these high mobility samples, is characterised by a resistivity that decreases exponentially with decreasing temperature. This behaviour, and the duality between resistivity and conductivity on the two sides of the transition, are very similar to that recently reported for high mobility Si-MOSFETs.",9708118v2 1999-07-08,High-Tc Superconductors in Applied Magnetic Fields Parallel to the CuO Planes: First Order Transition with Slow Onset of Resistivity,"The three dimensional uniformly frustrated XY model is used as a model of a high temperature superconductor in an applied magnetic field parallel to the CuO-planes. Through Monte Carlo simulations with anisotropy $\eta^2 = 10$ on large lattices we find evidence for a first order transition. Earlier simulations and theoretical treatments are discussed and the experimentally found smooth onset of resistivity is suggested to be due to a large potential barrier against vortex line motion above $T_c$ present for perfect alignment of the applied field.",9907118v1 2001-03-08,Experimental observation of Frohlich superconductivity in high magnetic fields,"Resistivity and irreversible magnetisation data taken within the high-magnetic-field CDWx phase of the quasi-two-dimensional organic metal alpha-(BEDT-TTF)2KHg(SCN)4 are shown to be consistent with a field-induced inhomogeneous superconducting phase. In-plane skin-depth measurements show that the resistive transition on entering the CDWx phase is both isotropic and representative of the bulk.",0103178v3 2001-07-26,Barkhausen-like conductance noise in polycrystalline high Tc superconductors immersed in a slowly varying magnetic field,"Analysis of the resistive transition of a polycristalline YBCO specimen produced by an a.c. magnetic field, reveals the presence of a large conductance noise signal which is repetitive over subsequent magnetization cycles. It is shown that the noise arises from avalanche effects produced by the simultaneous resistive transition of large groups of weak links. Owing to its repeatability, the noise signal may be considered a sort of signature of the weak links critical current distribution, making it an interesting new tool for the study of high Tc ceramic superconductors, as reported measurements of noise hysteresis show.",0107543v1 2003-09-05,Magnetothermal Conductivity of Highly Oriented Pyrolytic Graphite in the Quantum Limit,"We report on the magnetic field (0T$ \le B \le 9$T) dependence of the longitudinal thermal conductivity $\kappa(T,B)$ of highly oriented pyrolytic graphite in the temperature range 5 K $\le T\le$ 20 K for fields parallel to the $c-$axis. We show that $\kappa(T,B)$ shows large oscillations in the high-field region (B > 2 T) where clear signs of the Quantum-Hall effect are observed in the Hall resistance. With the measured longitudinal electrical resistivity we show that the Wiedemann-Franz law is violated in the high-field regime.",0309129v1 2005-11-08,Magneto-transport and divergent screening of driven two dimensional electron gas in high Landau levels,"In two dimensional electron system in magnetic fields such that the Fermi energy lies in high Landau levels and driven by microwave $ac$-field a divergence of the Coulomb screening due to the Ryzhii photocurrent is predicted. A model of magneto-transport with superposition of long range and short range disorders is introduced. In this model the larger is the gradient of the long range potential the smaller is the longitudinal conductivity/resistivity. As a consequence a qualitative theory of the recently discovered zero-resistance states is given.",0511195v1 2006-02-10,Quantum critical phase in BaVS$_3$,"We study the high-pressure metallic phase of high-purity single crystals of BaVS$_3$ by measuring the temperature, pressure, and magnetic field dependence of the resistivity. Above the critical pressure of $p_{\rm cr}=1.97$GPa an extended non-Fermi liquid $p-T$ regime emerges with resistivity exponent $1.5 \le n<2$, crossing over to a FL only around $p=2.7$GPa. A hysteretic feature indicates that close to the insulator--metal boundary, the system is magnetically ordered. Our findings reveal a close analogy between the extended partially ordered NFL state of non-conventional itinerant magnets and the corresponding state of BaVS$_3",0602262v1 2007-08-16,Pressure-induced Superconductivity in CaLi2,"A search for superconductivity has been carried out on the hexagonal polymorph of Laves-phase CaLi2, a compound for which Feng, Ashcroft, and Hoffmann predict highly anomalous behavior under pressure. No superconductivity is observed above 1.10 K at ambient pressure. However, high-pressure ac susceptibility and electrical resistivity studies to 81 GPa reveal bulk superconductivity in CaLi2 at temperatures as high as 13 K. The normal-state resistivity shows a dramatic increase with pressure.",0708.2117v2 2011-02-02,Higher order finite difference schemes for the magnetic induction equations with resistivity,"In this paper, we design high order accurate and stable finite difference schemes for the initial-boundary value problem, associated with the magnetic induction equation with resistivity. We use Summation-By-Parts (SBP) finite difference operators to approximate spatial derivatives and a Simultaneous Approximation Term (SAT) technique for implementing boundary conditions. The resulting schemes are shown to be energy stable. Various numerical experiments demonstrating both the stability and the high order of accuracy of the schemes are presented.",1102.0480v1 2011-10-10,Non-linear transport phenomena in a two-subband system,"We study non-linear transport phenomena in a high-mobility bilayer system with two closely spaced populated electronic subbands in a perpendicular magnetic field. For a moderate direct current excitation, we observe zero-differential-resistance states with a characteristic 1/B periodicity. We investigate, both experimentally and theoretically, the Hall field-induced resistance oscillations which modulate the high-frequency magneto-intersubband oscillations in our system if we increase the current. We also observe and describe the influence of direct current on the magnetoresistance in the presence of microwave irradiation.",1110.1953v1 2011-12-20,Phase of phonon-induced resistance oscillations in a high-mobility two-dimensional electron gas,"We report on experimental studies of magnetoresistance oscillations that originate from the resonant interaction of two-dimensional electrons with thermal transverse-acoustic phonons in very high-mobility GaAs/AlGaAs quantum wells. We find that the oscillation maxima consistently occur when a frequency of a phonon with twice the Fermi momentum exceeds an integer multiple of the cyclotron frequency. This observation is in contrast to to all previous experiments associating resistance maxima with magnetophonon resonance and its harmonics. Our experimentally obtained resonant condition is in excellent quantitative agreement with recent theoretical proposals.",1112.4766v1 2013-12-17,High-temperature thermoelectric properties of novel layered bismuth-sulfide LaO1-xFxBiS2,"We have investigated the high-temperature thermoelectric properties of the layered compound LaO1-xFxBiS2. The electrical resistivity of LaOBiS2 showed an anomalous behavior; a metal-semiconductor transition was observed around 270 K. It was found that the value of the electrical resistivity decreased with F substitution. The Seebeck coefficient decreased with increasing F concentration. The highest power factor of 1.9 W/cmK2 at 480 C was obtained for LaOBiS2.",1312.4694v1 2015-11-16,Spinless composite fermions in an ultra-high quality strained Ge quantum well,"We report on an observation of a fractional quantum Hall effect in an ultra-high quality two-dimensional hole gas hosted in a strained Ge quantum well. The Hall resistance reveals precisely quantized plateaus and vanishing longitudinal resistance at filling factors $\nu = 2/3, 4/3$ and $5/3$. From the temperature dependence around $\nu = 3/2$ we obtain the composite fermion mass of $m^\star \approx 0.4\,m_e$, where $m_e$ is the mass of a free electron. Owing to large Zeeman energy, all observed states are spin-polarized and can be described in terms of spinless composite fermions.",1511.05164v1 2016-02-18,Resistive method for measuring the disintegration speed of Prince Rupert's drops,"We have successfully applied the resistance grid technique to measure the disintegration speed in special type of glass objects, widely known as Prince Rupert's drops. We use a digital oscilloscope and a simple electrical circuit, glued to the surface of the drops, to detect the voltage changes, corresponding to the breaks in the specific parts of the drops. The results obtained using this method are in good qualitative and quantitative agreement with theoretical predictions and previously published data. Moreover, the proposed experimental setup doesn't include any expensive equipment (such as a high-speed camera) and can therefore be widely used in high schools and universities.",1602.06801v1 2016-05-30,Comparison of CMS Resistive Plate Chambers performance during LHC RUN-1 and RUN-2,"The Resistive Plate Chambers detector system at the CMS experiment at the LHC provides robustness and redundancy to the muon trigger. A total of 1056 double-gap chambers cover the pseudo-rapidity region < 1.6. The main detector parameters and environmental conditions are constantly and closely monitored to achieve operational stability and high quality data in the harsh conditions of the second run period of the LHC with center-of-mass energy of 13 TeV. First results of overall detector stability with 2015 data and comparisons with data from the LHC RUN-1 period at 8 TeV are presented.",1605.09366v1 2017-03-01,Tunable Negative Differential Resistance in Planer Graphene Superlattice Resonant Tunneling Diode,"In this paper, we report on the controllable negative differential resistance (NDR) in a proposed planar graphene superlattice structure. High value of peak to valley ratio (PVR) is predicted. This is significant because of appearance of NDR with high PVR at low biases. Our finding is important since beside the other potential applications of the graphene, proposes implementation of the graphene based superlattice in electronic devices such as resonant tunneling diode and filters.",1703.00148v1 2019-01-09,Optical conductivity of granular aluminum films near the Mott metal-to-insulator transition,"We report measurements of the energy gap of granular aluminum films by THz spectroscopy. We find that as the grains progressively decouple, the coupling ratio $2\Delta(0)/k_{B}T_{c}$ increases above the BCS weak coupling ratio $3.53$, and reaches values consistent with an approach to BCS-BEC crossover for the high resistivity samples, expected from the short coherence length. The Mattis-Bardeen theory describes remarkably well the behavior of $\sigma_{1,s}/\sigma_{1,n}$ for all samples up to very high normal state resistivities.",1901.02814v2 2020-05-26,CMS RPC Activities During LHC LS-2,"The second LHC long shutdown period (LS2) is an important opportunity for the CMS Resistive Plate Chambers (RPC) to complete their consolidation and upgrade projects. The consolidation includes detector maintenance for gas tightness, HV (high voltage), LV (low voltage) and slow control operation. All services for the RPC Phase-2 upgrade, namely RE3/1 and RE4/1, were anticipated for installation to LS2. This paper summarises the RPC system maintenance and upgrade activities.",2005.12534v1 2021-02-27,Spin polarization dynamics in the Bjorken-expanding resistive MHD background,"Evolution of spin polarization in the presence of external electric field is studied for collision energies $\sqrt{s_{\rm NN}}=27\,{\rm GeV}$ and $\sqrt{s_{\rm NN}}=200\,{\rm GeV}$. The numerical analysis is done in the perfect-fluid Bjorken-expanding resistive magnetohydrodynamic background and novel results are reported. In particular, we show that the electric field plays a significant role in the competition between expansion and dissipation.",2103.02592v2 2023-01-01,High-resistivity niobium nitride films for unity-efficiency SMSPDs at telecom wavelengths and beyond,"The sensitive element of superconducting single-photon detectors made in the form of a microstrip promise to resolve significant limitations caused by their typical design. However, attention should be paid to the problem of deterioration of the detection efficiency of devices with an increase of the width of the superconducting strip from nano- to microscale. This article demonstrates a possibility of achieving highly saturated detection efficiency of superconducting microstrip single-photon detectors by using high-resistivity niobium nitride films. The approach opens the way for employing fundamentally improved experimental devices.",2301.00400v1 2023-08-18,Resistive relativistic MHD simulations of astrophysical jets,"Aims. The main goal of the present paper is to provide the first systematic numerical study of the propagation of astrophysical relativistic jets, in the context of high-resolution shock-capturing resistive relativistic magnetohydrodynamics (RRMHD) simulations. We aim at investigating different values and models for the plasma resistivity coefficient, and at assessing their impact on the level of turbulence, the formation of current sheets and reconnection plasmoids, the electromagnetic energy content, and the dissipated power. Methods. We use the PLUTO code for simulations and we assume an axisymmetric setup for jets, endowed with both poloidal and toroidal magnetic fields, and propagating in a uniform magnetized medium. The gas is assumed to be characterized by a realistic Synge-like equation of state (Taub equation), appropriate for such type of astrophysical jets. The Taub equation is combined here for the first time with the Implicit-Explicit Runge-Kutta time-stepping procedure, as required in RRMHD simulations. Results. The main result is that turbulence is clearly suppressed for the highest values of resistivity (low Lundquist numbers), current sheets are broader, and plasmoids are barely present, while for low values of resistivity results are very similar to ideal runs, where dissipation is purely numerical. We find that recipes employing a variable resistivity based on the advection of a jet tracer or on the assumption of a uniform Lundquist number improve on the use of a constant coefficient and are probably more realistic, preserving the development of turbulence and of sharp current sheets, possible sites for the acceleration of the non-thermal particles producing the observed high-energy emission.",2308.09477v2 2015-10-23,Origin of the turn-on temperature behavior in WTe$_2$,"A hallmark of materials with extremely large magnetoresistance (XMR) is the transformative 'turn-on' temperature behavior: when the applied magnetic field $H$ is above certain value, the resistivity versus temperature $\rho(T)$ curve shows a minimum at a field dependent temperature $T^*$, which has been interpreted as a magnetic-field-driven metal-insulator transition or attributed to an electronic structure change. Here, we demonstrate that $\rho(T)$ curves with turn-on behavior in the newly discovered XMR material WTe$_2$ can be scaled as MR $\sim(H/\rho_0)^m$ with $m\approx 2$ and $\rho_0$ being the resistivity at zero-field. We obtained experimentally and also derived from the observed scaling the magnetic field dependence of the turn-on temperature $T^* \sim (H-H_c)^\nu$ with $\nu \approx 1/2$, which was earlier used as evidence for a predicted metal-insulator transition. The scaling also leads to a simple quantitative expression for the resistivity $\rho^* \approx 2 \rho_0$ at the onset of the XMR behavior, which fits the data remarkably well. These results exclude the possible existence of a magnetic-field-driven metal-insulator transition or significant contribution of an electronic structure change to the low-temperature XMR in WTe$_2$. This work resolves the origin of the turn-on behavior observed in several XMR materials and also provides a general route for a quantitative understanding of the temperature dependence of MR in both XMR and non-XMR materials.",1510.06976v2 2023-07-20,Nanoscale imaging of He-ion irradiation effects on amorphous TaO$_x$ toward electroforming-free neuromorphic functions,"Resistive switching in thin films has been widely studied in a broad range of materials. Yet the mechanisms behind electroresistive switching have been persistently difficult to decipher and control, in part due to their non-equilibrium nature. Here, we demonstrate new experimental approaches that can probe resistive switching phenomena, utilizing amorphous TaO$_x$ as a model material system. Specifically, we apply Scanning Microwave Impedance Microscopy (sMIM) and cathodoluminescence (CL) microscopy as direct probes of conductance and electronic structure, respectively. These methods provide direct evidence of the electronic state of TaO$_x$ despite its amorphous nature. For example CL identifies characteristic impurity levels in TaO$_x$, in agreement with first principles calculations. We applied these methods to investigate He-ion-beam irradiation as a path to activate conductivity of materials and enable electroforming-free control over resistive switching. However, we find that even though He-ions begin to modify the nature of bonds even at the lowest doses, the films conductive properties exhibit remarkable stability with large displacement damage and they are driven to metallic states only at the limit of structural decomposition. Finally, we show that electroforming in a nanoscale junction can be carried out with a dissipated power of < 20 nW, a much smaller value compared to earlier studies and one that minimizes irreversible structural modifications of the films. The multimodal approach described here provides a new framework toward the theory/experiment guided design and optimization of electroresistive materials.",2307.11189v1 1998-03-09,Negative Domain Wall Contribution to the Resistivity of Microfabricated Fe Wires,"The effect of domain walls on electron transport has been investigated in microfabricated Fe wires (0.65 to 20 $\mu m$ linewidths) with controlled stripe domains. Magnetoresistance (MR) measurements as a function of domain wall density, temperature and the angle of the applied field are used to determine the low field MR contributions due to conventional sources in ferromagnetic materials and that due to the erasure of domain walls. A negative domain wall contribution to the resistivity is found. This result is discussed in light of a recent theoretical study of the effect of domain walls on quantum transport.",9803102v1 1999-01-22,"Magnetoresistance, Micromagnetism, and Domain Wall Scattering in Epitaxial hcp Co Films","Large negative magnetoresistance (MR) observed in transport measurements of hcp Co films with stripe domains were recently reported and interpreted in terms of a novel domain wall (DW) scattering mechanism. Here detailed MR measurements, magnetic force microscopy, and micromagnetic calculations are combined to elucidate the origin of MR in this material. The large negative room temperature MR reported previously is shown to be due to ferromagnetic resistivity anisotropy. Measurements of the resistivity for currents parallel (CIW) and perpendicular to DWs (CPW) have been conducted as a function of temperature. Low temperature results show that any intrinsic effect of DWs scattering on MR of this material is very small compared to the anisotropic MR.",9901245v1 2001-10-12,Large Thermopower in Metallic Oxides: Misfit Cobaltites and Mangano-Ruthenates,"Two different kinds of metal transition oxides have been studied for their large thermopower values. The first one corresponds to the Tl-based misfit cobaltite which is a hole-doped metal. We demonstrate that the partial Bi-substitution for Tl in this phase induces an increase of the room temperature (RT) thermopower (TEP) value. Same result is obtained with the new Pb_{1/3}SrCoO_{3+delta} misfit corresponding to the Tl complete replacement by lead. Simultaneously, the T dependence of their resistivity exhibits a re-entrance below 70-90K where a large negative magnetoresistance is observed. Magnetic measurements reveal a strong interplay between spins and charges for this class of materials. Electron-doped (n-type) perovskite manganites are a second class of potential candidates for applications. In particular, the Ru^{4+/5+} substitution for Mn in the CaMnO_3 semi-conductor induces a drastic drop of the resistivity values. Metals with large RT TEP values and not too large thermal conductivities are generated. A comparison with best known materials, Bi_2Te_3 and NaCo_2O_4 is made.",0110270v1 2001-11-05,Large Thermoelectric Power Factor in TiS2 Crystal with Nearly Stoichiometric Composition,"A TiS$_{2}$ crystal with a layered structure was found to have a large thermoelectric power factor.The in-plane power factor $S^{2}/ \rho$ at 300 K is 37.1~$\mu$W/K$^{2}$cm with resistivity ($\rho$) of 1.7 m$\Omega$cm and thermopower ($S$) of -251~$\mu$V/K, and this value is comparable to that of the best thermoelectric material, Bi$_{2}$Te$_{3}$ alloy. The electrical resistivity shows both metallic and highly anisotropic behaviors, suggesting that the electronic structure of this TiS$_{2}$ crystal has a quasi-two-dimensional nature. The large thermoelectric response can be ascribed to the large density of state just above the Fermi energy and inter-valley scattering. In spite of the large power factor, the figure of merit, $ZT$ of TiS$_{2}$ is 0.16 at 300 K, because of relatively large thermal conductivity, 68~mW/Kcm. However, most of this value comes from reducible lattice contribution. Thus, $ZT$ can be improved by reducing lattice thermal conductivity, e.g., by introducing a rattling unit into the inter-layer sites.",0111063v1 2002-02-07,Resistivity extrema in double exchange ferromagnetic nondegenerate semiconductors,"A version of the magnetoimpurity theory of the colossal magnetoresistance materials suitable for the double exchange ferromagnetic nondegenerate semiconductors is presented. It provides an explanation of the nonmonotonic temperature dependence for the charge carrier density in them when it displays first a maximum and then a minimum, on increase in temperature. Respectively, the resistivity displays first a minimum and then a maximum. The theory is based on the relation between the charge carrier activation energy and the change in the magnon free energy caused by the ionization of an impurity. This is tantamount to the relation between the charge carrier density and the so called giant red shift of the optical absorption edge.",0202126v1 2002-10-11,On the residual resistivity near a two dimensional metamagnetic quantum critical point,"The behavior of the residual (impurity-dominated) resistivity is computed for a material near a two dimensional quantum critical point characterized by a divergent $q=0$ susceptibility. A singular renormalization of the amplitude for back-scattering of an electron off of a single impurity is found. When the correlation length of the quantum critical point exceeds the mean free path, the singular renormalization is found to convert the familiar `Altshuler-Aronov' logarithmic correction to the conductivity into a squared-logarithmic form. Impurities can induce unconventional Friedel oscillations, which may be observable in scanning tunnelling microscope experiments. Possible connections to the metamagnetic quantum critical end point recently proposed for the material $Sr_{3}Ru_{2}O_{7}$ are discussed.",0210260v1 2003-01-27,Semiconductive and Photoconductive Properties of the Single Molecule Magnets Mn12-Acetate and Fe8Br8,"Resistivity measurements are reported for single crystals of Mn12-Acetate and Fe8Br8. Both materials exhibit a semiconductor-like, thermally activated behavior over the 200-300 K range. The activation energy, Ea, obtained for Mn12-Acetate was 0.37 +/- 0.05 eV, which is to be contrasted with the value of 0.55 eV deduced from the earlier reported absorption edge measurements and the range of 0.3-1 eV from intramolecular density of states calculations, assuming 2Ea = Eg, the optical band gap. For Fe8Br8, Ea was measured as 0.73 +/- 0.1 eV, and is discussed in light of the available approximate band structure calculations. Some plausible pathways are indicated based on the crystal structures of both lattices. For Mn12-Acetate, we also measured photoconductivity in the visible range; the conductivity increased by a factor of about eight on increasing the photon energy from 632.8 nm (red) to 488 nm (blue). X-ray irradiation increased the resistivity, but Ea was insensitive to exposure.",0301515v1 2003-10-16,AC magnetic behavior of large grain magneto-resistive La0.78Ca0.22Mn0.90Ox materials,"We report a detailed set of AC magnetic measurements carried out on bulk large grain La-Ca-Mn-O samples extracted from a floating zone method-grown rod. Three samples with $La_{0.78}Ca_{0.22}Mn_{0.90}O_{x}$ stoichiometry but differing in their microstructure were investigated by electrical resistivity and AC susceptibility measurements: (i) a single grain sample, (ii) a sample containing two grains and (iii) a polycrystalline sample. We show that the superimposition of DC magnetic fields during AC magnetic susceptibility measurements is an efficient way for characterizing the magnetic transition of samples with different microstructures. Whereas both single grain and polycrystalline samples display a single susceptibility peak, an additional kink structure is observed in the case of the double grain sample. The temperature dependence of the AC susceptibility measured with superimposed DC magnetic fields is analyzed in the framework of second-order phase transition ideas. The relations between the critical exponents ($\beta + \gamma$ ~ 1.5, $\delta$ ~ 2.5) are found to be close to those of the mean-field model for all samples. This is attributed to the disordering caused by unoccupied Mn sites.",0310376v1 2004-01-16,Study of the SmBaCuO solid solutions decomposition and its possible role for changing critical current,"We studied thermochemical characteristics of the Sm1+xBa2-xCu3Oy single crystals by solution calorimetry. Dependences of formation enthalpies from samarium content were constructed. It was established that solid solutions on the bases of Sm123 could be decomposed both in inert and in oxygen atmosphere into different mixtures. We supposed that solid solutions decomposition could lead to increasing critical current density. We assumed from thermochemical data that Jc could be greater for samples prepared in oxygen than for samples synthesized in inert atmosphere. We confirmed these assumptions by comparison of obtained thermochemical data with transport properties measured in literature. We also investigated temperature dependences of resistance in the temperature range of 300-550 K during slow heating. As it was shown there was anomaly of resistance near 500 K. The origin of this anomaly was discussed.",0401277v1 2004-05-20,Tunnel Magneto-resistance in GaMnAs: going beyond Jullière formula,"The relation between tunnel magneto-resistance (TMR) and spin polarization is explored for GaMnAs/GaAlAs/GaMnAs structures where the carriers experience strong spin-orbit interactions. TMR is calculated using Landauer approach. The materials are described in the 6 band $\bf {k}\cdot \bf{p}$ model which includes spin orbit interaction. Ferromagnetism is described in the virtual crystal mean field approximations. Our results indicate that TMR is a function of of spin polarization and barrier thickness. As a result of the stong spin orbit interactions, TMR also depends on the the angle between current flow direction and the electrode magnetization. These results compromise the validity of Julliere formula.",0405473v2 2004-06-21,Nonquasiparticle states in half-metallic ferromagnets,"Anomalous magnetic and electronic properties of the half-metallic ferromagnets (HMF) have been discussed. The general conception of the HMF electronic structure which take into account the most important correlation effects from electron-magnon interactions, in particular, the spin-polaron effects, is presented. Special attention is paid to the so called non-quasiparticle (NQP) or incoherent states which are present in the gap near the Fermi level and can give considerable contributions to thermodynamic and transport properties. Prospects of experimental observation of the NQP states in core-level spectroscopy is discussed. Special features of transport properties of the HMF which are connected with the absence of one-magnon spin-flip scattering processes are investigated. The temperature and magnetic field dependences of resistivity in various regimes are calculated. It is shown that the NQP states can give a dominate contribution to the temperature dependence of the impurity-induced resistivity and in the tunnel junction conductivity. First principle calculations of the NQP-states for the prototype half-metallic material NiMnSb within the local-density approximation plus dynamical mean field theory (LDA+DMFT) are presented.",0406487v1 2004-08-24,Current-induced metallic behavior in Pr$_{0.5}$Ca$_{0.5}$MnO$_3$ thin films: competition between Joule heating and nonlinear conduction mechanism,"Thin films of Pr0.5Ca0.5MnO3 manganites exhibiting charge/orbital-ordered properties with colossal magnetoresistance have been synthesized by the pulsed laser deposition technique on both (100)-SrTiO3 and (100)-LaAlO3 substrates. The effects of current-induced metallic-behavior of the films are investigated as a function of the temperature and the magnetic field. Calculations based on a heat transfer model across the substrate, and our resistivity measurements reveal effects of Joule heating on charge transport over certain ranges of temperatures and magnetic fields. Our results also indicate that a nonlinear conduction, which cannot be explained by homogeneous Joule heating of the film, is observed when the material is less resistive (10-2 W.cm). The origin of this behavior is explained with a model based on local thermal instabilities associated with phase-separation mechanism and a change in the long range charge-ordered state.",0408512v1 2004-10-04,What does intrinsic tunnelling spectroscopy really examine?,"The out-of-plane current-voltage (I-V) characteristics of Bi2212 are studied in experimental environments of different heat transfer efficiency, allowing practical separation of intrinsic and extrinsic phenomena. {\it Intrinsic} (heating-free) response is Ohmic in the normal state of Bi2212, while its resistance, R=V/I, is found to be a good practical measure of the mean temperature of the sample in the overheated case. A self-heating model proposed for the latter case provides a qualitative and quantitative description of key findings of intrinsic tunnelling spectroscopy including (pseudo)gaps, quasiparticle and normal state resistances. The model also naturally explains the `superconducting' gap closure well below $T_c$ of the material as well as its survival at a magnetic field significantly exceeding $H_{c2}$. The generic shape of the individual branches of the brush-like part of I-V established under conditions of negligible overheating suggests a phase-slip origin of the so-called `intrinsic Josephson effect' (IJE).",0410069v1 2004-10-14,Carbon Nanotubes in Microelectronic Applications,"Carbon nanotubes with their outstanding electrical and mechanical properties are suggested as interconnect material of the future and as switching devices, which could outperform silicon devices. In this paper we will introduce nanotubes, specify the applications, where nanotubes can contribute to the advancement of Moore's law and show our progress of nanotube process integration in a microelectronic compatible way. The growth of single individual nanotubes at lithographically defined locations on whole wafers as a key requirement for the successful implementation of nanotubes is shown. In terms of nanotube transistors we propose a vertical nanotube transistor concept which outperforms the ITRS requirements for the year 2016. The performance is mainly limited by contact resistances, but by comparison with silicon devices we show that fabricated nanotube transistors already today exceed the values for transconductance, on-resistance and drive current of silicon devices.",0410360v1 2004-12-13,Unusual thermoelectric behavior of packed crystalline granular metals,"Loosely packed granular materials are intensively studied nowadays. Electrical and thermal transport properties should reflect the granular structure as well as intrinsic properties. We have compacted crystalline $CaAl$ based metallic grains and studied the electrical resistivity and the thermoelectric power as a function of temperature ($T$) from 15 to 300K. Both properties show three regimes as a function of temperature. It should be pointed out : (i) The electrical resistivity continuously decreases between 15 and 235 K (ii) with various dependences, e.g. $\simeq$ $T^{-3/4}$ at low $T$, while (iii) the thermoelectric power (TEP) is positive, (iv) shows a bump near 60K, and (v) presents a rather unusual square root of temperature dependence at low temperature. It is argued that these three regimes indicate a competition between geometric and thermal processes, - for which a theory seems to be missing in the case of TEP. The microchemical analysis results are also reported indicating a complex microstructure inherent to the phase diagram peritectic intricacies of this binary alloy.",0412323v1 2005-07-01,Resistivity memory effect in La(1-x)Sr(x)MnO(3),"During the study of magnetoresistivity in La(1-x)Ca(x)MnO(3) it was found that after cycling of the magnetic field, some kind of magnetic field memory effect was observed. For La0.5Ca0.5MnO3 after cycling of the magnetic field to 13T and back to zero, ""frozen"" magnetoresistivity decreases about 20 times comparing to zero field value, while for La(0.47)Ca(0.53)MnO(3) it is already about four orders of magnitude. This effect can be observed only for concentration region 0.45 < x < 0.55. In zero magnetic field, temperature dependence of resistivity ro(T) shows semiconducting-like behavior, while after magnetic field cycling it becomes metal-like. So it looks as we are dealing with magnetic field induced semiconductor (or dielectric) to metal transition. Such effect can be explained within phase-separation picture. In zero magnetic field material consists of antiferromagnetic matrix (insulating phase) and coexisting ferromagnetic, conducting phase. Magnetic field application causes ferromagnetic phase to form some kind of conducting channels which shunts semiconducting matrix phase. Such structure is preserved after reduction of magnetic field, leaving the material conducting.",0507018v2 2005-08-06,Modelling the 0.6 - 0.7 power law of permittivity and admittance frequency responses in random R-C networks,"The dielectric response of complex materials is characterized, in many cases, by a similar power law frequency dependence of both the real and the imaginary parts of their complex dielectric constants. In the admittance representation, this power law is often shown as the constant phase angle (CPA) response. Apparently, the power that characterizes many different systems, when expressed as the frequency dispersion of conductivity (the real part of admittance) is often found to be in the range of 0.6 - 0.7 or having frequency independent, constant phase angles (CPA) of about 54 - 63 deg. The model suggested here is based on series-parallel mixing of resistors' and capacitors' responses in a random R-C network. A geometric mean evaluation of the effective resistivity of conductors having a uniform distribution of resistivity is used. In contrast to models based on percolation arguments, the model suggested here can be applied to both 2D and 3D systems.",0508170v2 2005-10-14,Superconducting transition in disordered granular superconductors in magnetic fields,"Motivated by a recent argument that the superconducting (SC) transition field of three-dimensional (3D) disordered superconductors with granular structure in a nonzero magnetic field should lie above $H_{c2}(0)$ in low $T$ limit, the glass transition (or, in 2D, crossover) curve $H_g(T)$ of disordered quantum Josephson junction arrays is examined by incorporating SC fluctuations. It is found that the glass transition or crossover in the granular materials can be described on the same footing as the vortex-glass (VG) transition in amorphous-like (i.e., nongranular) materials. In most of 3D granular systems, the vanishing of resistivity upon cooling should occur even above $H_{c2}(0)$, while the corresponding sharp drop of the resistivity in 2D case may appear only below $H_{c2}$ as a result of an enhanced quantum fluctuation.",0510380v5 2005-11-19,"Transport, thermal and magnetic properties of RuSr_2(Gd_{1.5}Ce_{0.5})Cu_2O_{10-δ}, a magnetic superconductor","Resistivity, thermoelectric power, heat capacity and magnetization for samples of RuSr_2(Gd_{1.5}Ce_{0.5})Cu_{2}O_{10-\delta} were investigated in the temperature range 1.8-300 K with a magnetic field up to 8 T. The resistive transitions to the superconducting state are found to be determined by the inhomogeneous (granular) structure, characterized by the intragranular, T_{c0}, and intergranular, T_{cg}, transition temperatures. Heat capacity, C(T), shows a jump at the superconducting transition temperature T_{c0}\approx 37.5 K. A Schottky-like anomaly is found in C(T) below 20 K. This low temperature anomaly can be attributed to splitting of the ground term $^{8}S_{7/2}$ of paramagnetic Gd^{3+} ions by internal and external magnetic fields.",0511489v1 2007-03-28,Comparison between experiment and calculated band structures for DyN and SmN,"We investigate the electronic band structure of two of the rare-earth nitrides, DyN and SmN. Resistivity measurements imply that both materials have a semiconducting ground state, and both show resistivity anomalies coinciding with the magnetic transition, despite the different magnetic states in DyN and SmN. X-ray absorption and emission measurements are in excellent agreement with LSDA+U calculations, although for SmN the calculations predict a zero band gap.",0703740v3 2007-04-24,Impedance spectroscopy of epitaxial multiferroic thin films,"Temperature dependent impedance spectroscopy enables the many contributions to the dielectric and resistive properties of condensed matter to be deconvoluted and characterized separately. We have achieved this for multiferroic epitaxial thin films of BiFeO3 (BFO) and BiMnO3 (BMO), key examples of materials with strong magneto-electric coupling. We demonstrate that the true film capacitance of the epitaxial layers is similar to that of the electrode interface, making analysis of capacitance as a function of film thickness necessary to achieve deconvolution. We modeled non-Debye impedance response using Gaussian distributions of relaxation times and reveal that conventional resistivity measurements on multiferroic layers may be dominated by interface effects. Thermally activated charge transport models yielded activation energies of 0.60 eV +- 0.05 eV (BFO) and 0.25 eV +- 0.03 eV (BMO), which is consistent with conduction dominated by oxygen vacancies (BFO) and electron hopping (BMO). The intrinsic film dielectric constants were determined to be 320 +- 75 (BFO) and 450 +- 100 (BMO).",0704.3262v1 2007-08-09,Carbon nanotube array vias for interconnect applications,"The material and electrical properties of the CNT single vias and array vias grown by microwave plasma-enhanced chemical vapor deposition were investigated. The diameters of multiwall carbon nanotubes (MWNTs) grown on the bottom electrode of Ta decrease with increasing pretreatment power and substrate temperature while the effects of the growth power and methane flow ratio are insignificant The decrease of CNT diameters leads to the decrease of the CNT via diode devices. The increase of growth power enhances the CNT graphitization degree and thue the conductivity of CNT via diode devices. In the same via region, the MWNT diode resistances of the array vias are lower than those of the single vias. The MWNT diode resistances on the bottom electrode of titanium are lower than those on the bottom electrode of tantalum. It may be attributed to the smaller tube diameters on the bottom electrode of Ti and the work function difference between Ta and Ti films with respect to the work function of CNTs.",0708.1298v1 2007-08-14,Suspension of Nanoparticles in SU-8 and Characterization of Nanocomposite Properties,"Gold nanospheres, single wall carbon nanotubes (SWNT), and diamonoids were phyically incorporated into the negative photoresist SU-8. the mixtures were spin cast onto silicon or aluminium coated silicon wafers. ASTM standard D638 tensile specimens were lithographically patterned in the materials and then released from the substrate using Microchem'Omnicoat or an anodic metal dissolution process. the residual stresses, elastic moduli, and viscosity of the SU-8. Resistivity measurements of SU-8/SWNT nanocomposites were also investigates. We found the effective modulus and viscosity of the SU-8 test specimens decreases with the addition of diamantane and SWNTs. Additionally, the SU-8/SWNT nanocomposites showed changes in resistivity with increased strain, suggesting a gauge factor for the 1 wt% SU-8/SWNT nanocomposite of approximately 2-4.",0708.1822v1 2007-12-07,Field Tuned Superconductor to Insulator Transitions in an Amorphous Film with an Imposed Multiply Connected Geometry,"We have observed multiple magnetic field driven superconductor to insulator transitions (SIT) in amorphous Bi films perforated with a nano-honeycomb (NHC) array of holes. The period of the magneto-resistance, H=H_M=h/2eS where S is the area of a unit cell of holes, indicates the field driven transitions are boson dominated. The field-dependent resistance follows R(T)=R_0(H)exp(T_0(H)/T) on both sides of the transition so that the evolution between these states is controlled by the vanishing of T_0 to0. We compare our results to the thickness driven transition in NHC films and the field driven transitions in unpatterned Bi films, other materials, and Josephson junction arrays. Our results suggest a structural source for similar behavior found in some materials and that despite the clear bosonic nature of the SITs, quasiparticle degrees of freedom likely also play an important part in the evolution of the SIT.",0712.1076v1 2008-07-02,Nano Imprint Lithography on Silica Sol-gels: a simple route to sequential patterning,"Since the pioneering work of S.Y. Chou et al.[1] Nano Imprint Lithography (NIL) has emerged as a promising technique for surface patterning, opening for numerous applications ranging from nanophotonics[2] to microfluidics[3]. NIL basically consists in the stamping of deformable surfaces or films. Preferred materials are thermoplastics[4] and UV curable resists[5]. So far, most papers report on single imprinting methods for which the same surface is imprinted only once. In the present paper, we report the imprinting of square silica structures from simple line gratings and demonstrate how the specific thermo-rheological behavior of ICSG resists can be harnessed to form complex structures by sequential imprinting at low pressures.",0807.0378v1 2009-01-09,Stability of a Charged Particle Beam in a Resistive Plasma Channel,"A self-focusing of a coasting relativistic beam in a plasma channel that is confined by an external magnetic field is studied as a means of reconditioning the beam emerging from a beam injector [a radio frequency quadrupole (RFQ)] for a linac. A detailed study of the beam stability in the self-focused beam has been carried out. In order to explain beam filaments and the resistive hose instability in a unified way, we treat all the azimuthal modes in the derivation of the dispersion relation in a finite plasma channel that exhibit many unstable modes, which are classified by Weinberg's scheme [Steven Weinberg, J. Math. 8, 614 (1967)].",0901.1167v2 2009-07-21,"Anomalous transport properties of the halfmetallic ferromagnets Co2TiSi, Co2TiGe, and Co2TiSn","In this work the theoretical and experimental investigations of Co2TiZ (Z = Si, Ge, or Sn) compounds are reported. Half-metallic ferromagnetism is predicted for all three compounds with only two bands crossing the Fermi energy in the majority channel. The magnetic moments fulfill the Slater-Pauling rule and the Curie temperatures are well above room temperature. All compounds show a metallic like resistivity for low temperatures up to their Curie temperature, above the resistivity changes to semiconducting like behavior. A large negative magnetoresistance of 55% is observed for Co2TiSn at room temperature in an applied magnetic field of 4T which is comparable to the large negative magnetoresistances of the manganites. The Seebeck coefficients are negative for all three compounds and reach their maximum values at their respective Curie temperatures and stay almost constant up to 950 K. The highest value achieved is -52muV/K m for Co2TiSn which is large for a metal. The combination of half-metallicity and the constant large Seebeck coefficient over a wide temperature range makes these compounds interesting materials for thermoelectric applications and further spincaloric investigations.",0907.3562v1 2009-08-27,"A low field technique for measuring magnetic and magneto-resistance anisotropy coefficients applied to (Ga,Mn)As","We demonstrate a simple, low cost, magneto-transport method for rapidly characterizing the magnetic anisotropy and anisotropic magneto-resistance (AMR) of ferromagnetic devices with uniaxial magnetic anisotropy. This transport technique is the analogue of magnetic susceptibility measurements of bulk material but is applicable to very small samples with low total moment. The technique is used to characterize devices fabricated from the dilute magnetic semiconductor (Ga,Mn)As. The technique allows us to probe the behavior of the parameters close to the Curie temperature, in the limit of the applied magnetic field tending to zero. This avoids the complications arising from the presence of paramagnetism.",0908.3960v1 2010-01-20,Robust charge and magnetic order under electric field and current in the multiferroic LuFe(2)O(4),"We performed elastic neutron scattering measurements on the charge- and magnetically-ordered multiferroic material LuFe(2)O(4). An external electric field along the [001] direction with strength up to 20 kV/cm applied at low temperature (~100 K) does not affect either the charge or magnetic structure. At higher temperatures (~360 K), before the transition to three-dimensional charge-ordered state, the resistivity of the sample is low, and an electric current was applied instead. A reduction of the charge and magnetic peak intensities occurs when the sample is cooled under a constant electric current. However, after calibrating the real sample temperature using its own resistance-temperature curve, we show that the actual sample temperature is higher than the thermometer readings, and the ""intensity reduction"" is entirely due to internal sample heating by the applied current. Our results suggest that the charge and magnetic orders in LuFe(2)O(4) are unaffected by the application of external electric field/current, and previously observed electric field/current effects can be naturally explained by internal sample heating.",1001.3611v2 2010-10-07,Compensation-dependence of magnetic and electrical properties in Ga1-xMnxP,"We demonstrate the control of the hole concentration in Ga1-xMnxP over a wide range by introducing compensating vacancies. The resulting evolution of the Curie temperature from 51 K to 7.5 K is remarkably similar to that observed in Ga1-xMnxAs despite the dramatically different character of hole transport between the two material systems. The highly localized nature of holes in Ga1-xMnxP is reflected in the accompanying increase in resistivity by many orders of magnitude. Based on variable-temperature resistivity data we present a general picture for hole conduction in which variable-range hopping is the dominant transport mechanism in the presence of compensation.",1010.1368v2 2011-02-04,Low-Frequency Current Fluctuations in Graphene-like Exfoliated Thin-Films of Topological Insulators,"We report on the low-frequency current fluctuations and electronic noise in thin-films made of bismuth selenide topological insulators. The films were prepared via the graphene-like mechanical exfoliation and used as the current conducting channels in the four- and two-contact devices. Analysis of the resistance dependence on the film thickness indicates that the surface contribution to conductance is dominant in our samples. It was established that the current fluctuations have the noise spectrum close to the pure 1/f in the frequency range from 1 to 10 kHz (f is the frequency). The relative noise amplitude S/I^2 for the examined films was increasing from ~5x10^-8 to 5x10^-6 (1/Hz) as the resistance of the channels varied from ~10^3 to 10^5 Ohms. The obtained noise data is important for understanding electron transport through the surface and volume of topological insulators, and proposed applications of this class of materials.",1102.0961v1 2011-05-04,Sondheimer Oscillation as a Fingerprint of Surface Dirac Fermions,"Topological states of matter challenge the paradigm of symmetry breaking, characterized by gapless boundary modes and protected by the topological property of the ground state. Recently, angle-resolved photoemission spectroscopy (ARPES) has revealed that semiconductors of Bi$_{2}$Se$_{3}$ and Bi$_{2}$Te$_{3}$ belong to such a class of materials. Here, we present undisputable evidence for the existence of gapless surface Dirac fermions from transport in Bi$_{2}$Te$_{3}$. We observe Sondheimer oscillation in magnetoresistance (MR). This oscillation originates from the quantization of motion due to the confinement of electrons within the surface layer. Based on Sondheimer's transport theory, we determine the thickness of the surface state from the oscillation data. In addition, we uncover the topological nature of the surface state, fitting consistently both the non-oscillatory part of MR and the Hall resistance. The side-jump contribution turns out to dominate around 1 T in Hall resistance while the Berry-curvature effect dominates in 3 T $\sim$ 4 T.",1105.0731v1 2011-07-05,Evidence for filamentary superconductivity nucleated at antiphase domain walls in antiferromagnetic CaFe$_2$As$_2$,"Resistivity, magnetization and microscopic $^{75}$As nuclear magnetic resonance (NMR) measurements in the antiferromagnetically ordered state of the iron-based superconductor parent material CaFe$_2$As$_2$ exhibit anomalous features that are consistent with the collective freezing of domain walls. Below $T^*\approx 10$ K, the resistivity exhibits a peak and downturn, the bulk magnetization exhibits a sharp increase, and $^{75}$As NMR measurements reveal the presence of slow fluctuations of the hyperfine field. These features in both the charge and spin response are strongly field dependent, are fully suppressed by $H^*\approx 15$ T, and suggest the presence of filamentary superconductivity nucleated at the antiphase domain walls in this material.",1107.0904v2 2011-08-22,Ferromagnetic Quantum Criticality in the Quasi-One-Dimensional Heavy Fermion Metal YbNi4P2,"We present a new Kondo-lattice system, YbNi4P2, which is a clean heavy-fermion metal with a severely reduced ferromagnetic ordering temperature at T_C=0.17K, evidenced by distinct anomalies in susceptibility, specific-heat, and resistivity measurements. The ferromagnetic nature of the transition, with only a small ordered moment of ~0.05mu_B, is established by a diverging susceptibility at T_C with huge absolute values in the ferromagnetically ordered state, severely reduced by small magnetic fields. Furthermore, YbNi4P2 is a stoichiometric system with a quasi-one-dimensional crystal and electronic structure and strong correlation effects which dominate the low temperature properties. This is reflected by a stronger-than-logarithmically diverging Sommerfeld coefficient and a linear-in-T resistivity above T_C which cannot be explained by any current theoretical predictions. These exciting characteristics are unique among all correlated electron systems and make this an interesting material for further in-depth investigations.",1108.4274v1 2012-10-18,Observation of a Large Photo-response in a Single Nanowire (Diameter ~30 nm) of Charge Transfer Complex Cu:TCNQ,"We report for the first time large photoresponse in a single NW of the charge transfer complex Cu:TCNQ. We fabricate a metal-semiconductor-metal device with a single NW and focus ion beam deposited Pt. We observe large photocurrent even at zero bias. The spectral dependence of the photoresponse follows the main absorption at ~ 405 nm which has the primarily responsible for photogenerated carriers. We have quantitatively analyzed the bias dependent photocurrent by a model of two back to back Schottky diodes connected by a series resistance. The observation shows that the large photoresponse of the device primarily occurs due to the reduction of the barrier at the contact regions due to illumination along with the photoconductive contribution. There is also a bias driven reduction of the nanowire resistance that is a unique feature for the material.",1210.5207v1 2013-01-16,Huge field-effect surface charge injection and conductance modulation in metallic thin films by electrochemical gating,"The field-effect technique, popular thanks to its application in common field-effect transistors, is here applied to metallic thin films by using as a dielectric a novel polymer electrolyte solution. The maximum injected surface charge, determined by a suitable modification of a classic method of electrochemistry called double-step chronocoulometry, reached some units in 10^15 charges/cm^2. At room temperature, relative variations of resistance up to 8%, 1.9% and 1.6% were observed in the case of gold, silver and copper, respectively and, if the films are thick enough (> 25 nm), results can be nicely explained within a free-electron model with parallel resistive channels. The huge charge injections achieved make this particular field-effect technique very promising for a vast variety of materials such as unconventional superconductors, graphene and 2D-like materials.",1301.3769v1 2013-02-05,Scaling of Non-Saturating MR and quantum oscillations in pristine and ion-implanted HOPG,"A wide variety of resistive and field dependent behaviors have been previously observed in both doped and non-doped Highly Oriented Pyrolytic Graphite (HOPG). We find HOPG samples to vary significantly in their temperature dependent resistances, even between portions taken from the same sample, yet they exhibit consistent non-saturating magnetoresistance (MR). The scaling behavior of the MR is shown to be characteristic of a model based on the Hall effect in granular materials. In addition to the large, field-linear MR, all samples exhibit Shubnikov-de Haas (SdH) oscillations. Additional samples were doped via ion-implantation by boron and phosphorous, but show no signs of superconductivity nor any systematic change in their magnetoresistive behavior. Analysis of the SdH data gives a 2D carrier density in agreement with previous results, and a large mean-free path relative to crystallite size, even in samples with thin ion-implanted surface layers.",1302.1229v1 2013-02-07,Thermoelectromotive force of hafnium at plastic deformation in regime of creep at temperature of 300 K,"The thermoelectromotive force and electrical resistivity of the polycrystalline hafnium (Hf) with the grain size of 10 {\mu}m during the process of plastic deformation in the regime of creep at the temperature of 300 K are precisely measured. It is shown that the thermoelectromotive force depends on the deformation mechanism nature, because of the changing magnitude of the electrons scattering on the different structural defects in the hafnium crystal lattice at the deformation process. The main research conclusion is that the method of thermoelectromotive force measurements is more informative, comparing to the method of electric resistivity measurements in the process of accurate characterization of the hafnium.",1302.1784v1 2013-03-11,Nanobatteries in redox-based resistive switches require extension of memristor theory,"Redox-based nanoionic resistive memory cells (ReRAMs) are one of the most promising emerging nano-devices for future information technology with applications for memory, logic and neuromorphic computing. Recently, the serendipitous discovery of the link between ReRAMs and memristors and memristive devices has further intensified the research in this field. Here we show on both a theoretical and an experimental level that nanoionic-type memristive elements are inherently controlled by non-equilibrium states resulting in a nanobattery. As a result the memristor theory must be extended to fit the observed non zerocrossing I-V characteristics. The initial electromotive force of the nanobattery depends on the chemistry and the transport properties of the materials system but can also be introduced during ReRAM cell operations. The emf has a strong impact on the dynamic behaviour of nanoscale memories, and thus, its control is one of the key factors for future device development and accurate modelling.",1303.2589v1 2013-07-02,Non-volatile ferroelastic switching of the Verwey transition and resistivity of epitaxial Fe3O4/PMN-PT (011),"A central goal of electronics based on correlated materials or 'Mottronics' is the ability to switch between distinct collective states with a control voltage. Small changes in structure and charge density near a transition can tip the balance between competing phases, leading to dramatic changes in electronic and magnetic properties. In this work, we demonstrate that an electric field induced two-step ferroelastic switching pathway in (011) oriented 0.71Pb(Mg1/3Nb2/3)O3-0.29PbTiO3 (PMN-PT) substrates can be used to tune the Verwey metal-insulator transition in epitaxial Fe3O4 films in a stable and reversible manner. We also observe robust non-volatile resistance switching in Fe3O4 up to room temperature, driven by ferroelastic strain. These results provides a framework for realizing non-volatile and reversible tuning of order parameters coupled to lattice-strain in epitaxial oxide heterostructures over a broad range of temperatures, with potential device applications.",1307.0838v1 2014-06-01,Effect of carrier concentration on magnetism and magnetic order in the pyrochlore iridates,"We present resistivity, magnetization, and zero field muon spin relaxation ($\mu$SR) data for the pyrochlore iridate materials Nd$_{2-x}$Ca$_{x}$Ir$_{2}$O$_{7}$ ($x = 0, 0.06$, and $0.10$) and Sm$_2$Ir$_2$O$_7$. While Nd$_{2}$Ir$_{2}$O$_{7}$ (Nd227) is weakly conducting, Sm$_{2}$Ir$_{2}$O$_{7}$ (Sm227) has slowly diverging resistivity at low temperature. Nd227 and Sm227 exhibit magnetic anomalies at $T_{M} = 105 K$ and $137 K$, respectively. However, zero-field $\mu$SR measurements show that long-range magnetic order of the Ir$^{4+}$ sublattice sets in at much lower temperatures ($T_{LRO} \sim 8 K$ for Nd227 and $70 K$ for Sm227); both materials show heavily damped muon precession with a characteristic frequency near 9 MHz. The magnetic anomaly at $T_{M}$ in Nd227 is not significantly affected by the introduction of hole carriers by Ca-substitution in the conducting Nd$_{2-x}$Ca$_{x}$Ir$_{2}$O$_{7}$ samples, but the muon precession is fully suppressed for both.",1406.0194v1 2014-10-07,Thickness Scaling Effect on Interfacial Barrier and Electrical Contact to Two-Dimensional MoS2 Layers,"Understanding the interfacial electrical properties between metallic electrodes and low dimensional semiconductors is essential for both fundamental science and practical applications. Here we report the observation of thickness reduction induced crossover of electrical contact at Au/MoS2 interfaces. For MoS2 thicker than 5 layers, the contact resistivity slightly decreases with reducing MoS2 thickness. By contrast, the contact resistivity sharply increases with reducing MoS2 thickness below 5 layers, mainly governed by the quantum confinement effect. It is found that the interfacial potential barrier can be finely tailored from 0.3 to 0.6 eV by merely varying MoS2 thickness. A full evolution diagram of energy level alignment is also drawn to elucidate the thickness scaling effect. The finding of tailoring interfacial properties with channel thickness represents a useful approach controlling the metal/semiconductor interfaces which may result in conceptually innovative functionalities.",1410.1943v2 2015-03-04,Observation of the chiral anomaly induced negative magneto-resistance in 3D Weyl semi-metal TaAs,"Weyl semi-metal is the three dimensional analog of graphene. According to the quantum field theory, the appearance of Weyl points near the Fermi level will cause novel transport phenomena related to chiral anomaly. In the present paper, we report the first experimental evidence for the long-anticipated negative magneto-resistance generated by the chiral anomaly in a newly predicted time-reversal invariant Weyl semi-metal material TaAs. Clear Shubnikov de Haas oscillations (SdH) have been detected starting from very weak magnetic field. Analysis of the SdH peaks gives the Berry phase accumulated along the cyclotron orbits to be {\pi}, indicating the existence of Weyl points.",1503.01304v1 2015-03-12,"Shubnikov-de Haas oscillations, weak antilocalization effect and large linear magnetoresistance in the putative topological superconductor LuPdBi","We present electronic transport and magnetic properties of single crystals of semimetallic half-Heusler phase LuPdBi, having theoretically predicted band inversion requisite for nontrivial topological properties. The compound exhibits superconductivity below a critical temperature $T_{\rm c}=1.8\,$K, with a zero-temperature upper critical field $B_{\rm c2}\approx2.3\,$T. Although superconducting state is clearly reflected in the electrical resistivity and magnetic susceptibility data, no corresponding anomaly can be seen in the specific heat. Temperature dependence of the electrical resistivity suggests existence of two parallel conduction channels: metallic and semiconducting, with the latter making negligible contribution at low temperatures. The magnetoresistance is huge and clearly shows a weak antilocalization effect in small magnetic fields. Above about 1.5 T, the magnetoresistance becomes linear and does not saturate in fields up to 9 T. The linear magnetoresistance is observed up to room temperature. Below 10 K, it is accompanied by Shubnikov-de Haas oscillations. Their analysis reveals charge carriers with effective mass of $0.06\,m_e$ and a Berry phase very close to $\pi$, expected for Dirac-fermion surface states, thus corroborating topological nature of the material.",1503.03697v1 2015-11-17,"Microstructure, mechanical properties and corrosion of friction stir welded 6061 Aluminum Alloy","The microstructure, mechanical properties, and corrosion behavior of friction stir welded (FSW) AA6061 aluminum alloys were investigated. Dynamic recrystallized structures were observed and grain sizes of nugget zone (NZ), thermomechanically-affected zone (TMAZ), heat-affected zone (HAZ), and base material (BM) were different. Hardness test indicated that the minimum and maximum hardness values wereobtained in the HAZ and BM, respectively. Tensile results showed that fracture occurred in the relatively weak regions in between TMAZ and HAZ. Polarization tests illustrated that the FSW process improved the corrosion resistance of AA6061-AA6061 and the HAZ had better corrosion resistance than other regions. Raman characterizations revealed that aluminum hydroxide was the main corrosion product formed on Al after immersion experiments. Intergranular attack was observed in the NZ and downside by scanning electron microscopy.",1511.05507v1 2015-11-20,Transmission conditions for thin curvilinear close to circular heat-resistant interphases in composite ceramics,"This paper considers the problem of heat transfer in a composite ceramic material where the structural elements are bonded to the matrix via a thin heat resistant adhesive layer. The layer has the form of a circular ring or close to it. Using an asymptotic approach, the interphase is modeled by an infinitesimal imperfect interface, preserving the main features of the temperature fields around the interphase, and allowing a significant simplification where FEM analysis is concerned. The nonlinear transmission conditions that accompany such an imperfect interface are evaluated, and their accuracy is verified by means of dedicated analytical examples as well as carefully designed FEM simulations. The interphases of various geometries are analysed, with an emphasis on the influence of the curvature of their boundaries on the accuracy of the evaluated conditions. Numerical results demonstrate the benefits of the approach and its limitations.",1511.06630v2 2015-11-29,Ultrafast electron-phonon-magnon interactions at noble metal-ferromagnet interfaces,"Ultrafast optical excitation of gold-cobalt bilayers triggers the nontrivial interplay between the electronic, acoustic, and magnetic degrees of freedom. Laser-heated electrons generated at the gold-air interface diffuse through the layer of gold and strongly overheat the lattice in cobalt resulting in the emission of ultrashort acoustic pulses and generation of exchange-coupled magnons. Time-resolved optical measurements allow for extracting the thermal boundary (Kapitza) resistances at metal/metal interfaces and the hot electron diffusion length in ferromagnetic materials. Both the experimental data and the analytical treatment of the two-temperature model reveal the role of the Kapitza resistance in transient lattice overheating.",1511.09060v3 2016-04-05,Gap state charge induced spin-dependent negative differential resistance in tunnel junctions,"We propose and demonstrate through first-principles calculation a new spin-dependent negative differential resistance (NDR) mechanism in magnetic tunnel junctions (MTJ) with cubic cation disordered crystals (CCDC) AlO$_x$ or Mg$_{1-x}$Al$_x$O as barrier materials. The CCDC is a class of insulators whose band gap can be changed by cation doping. The gap becomes arched in an ultrathin layer due to the space charge formed from metal-induced gap states. With an appropriate combination of an arched gap and a bias voltage, NDR can be produced in either spin channel. This mechanism is applicable to 2D and 3D ultrathin junctions with a sufficiently small band gap that forms a large space charge. It provides a new way of controlling the spin-dependent transport in spintronic devices by an electric field. A generalized Simmons formula for tunneling current through junction with an arched gap is derived to show the general conditions under which ultrathin junctions may exhibit NDR.",1604.01364v1 2016-05-12,Thermoelectric performance of spin Seebeck effect in Fe3O4/Pt-based thin film heterostructures,"We report a systematic study on the thermoelectric performance of spin Seebeck devices based on Fe3O4/Pt junction systems. We explore two types of device geometries: a spin Hall thermopile and spin Seebeck multilayer structures. The spin Hall thermopile increases the sensitivity of the spin Seebeck effect, while the increase in the sample internal resistance has a detrimental effect on the output power. We found that the spin Seebeck multilayers can overcome this limitation since the multilayers exhibit the enhancement of the thermoelectric voltage and the reduction of the internal resistance simultaneously, therefore resulting in significant power enhancement. This result demonstrates that the multilayer structures are useful for improving the thermoelectric performance of the spin Seebeck effect.",1605.03752v1 2016-06-15,Response of Carbon Nanotube (CNT) Ply Subjected to a Pulsed Magnetic Field,"In this study, the possible deformation of a single Carbon Nanotube (CNT) ply subjected to a pulsed magnetic field was investigated. In all tests the capacitor bank was charged to 6kJ of energy. A Photon Doppler Velocimetry (PDV) system was used to measure velocity or displacement of the CNT ply during the experiments. The resistance of the CNT ply was measured using four-point probe technique before and after the experiments. Preliminary results show that the single CNT plies do not permanently deform in response to the pulsed magnetic fields. However, they can be displaced, either by themselves a small amount (0.6mm) or by a large amount using a driver material. Also, the resistance of the CNT plies may increase or decrease depends on the lay-out (i.e., yarn) and current flow directions.",1606.04893v2 2016-07-28,A 3D dislocation dynamics analysis of the size effect on the strength of [111] LiF micropillars at 300K and 600K,"The mechanical behavior in compression of [111] LiF micropillars with diameters in the range 0.5 $\mu$m to 2.0 $\mu$m was analyzed by means of discrete dislocation dynamics at ambient and elevated temperature. The dislocation velocity was obtained from the Peach-Koehler force acting on the dislocation segments from a thermally-activated model that accounted for the influence of temperature on the lattice resistance. A size effect of the type ""smaller is stronger"" was predicted by the simulations, which was in quantitative agreement with previous experimental results by the authors \cite{SWC14}. The contribution of the different physical deformation mechanisms to the size effect (namely, nucleation of dislocations, dislocation exhaustion and forest hardening) could be ascertained from the simulations and the dominant deformation mode could be assessed as a function of the specimen size and temperature. These results shed light into the complex interaction among size, lattice resistance and dislocation mobility in the mechanical behavior of $\mu$m-sized single crystals.",1607.08642v1 2016-11-20,Uniform Benchmarking of Low Voltage Van Der Waals FETs,"Monolayer MoS2, MoSe2, MoTe2, WS2, WSe2, and black phosphorous field effect transistors (FETs) operating in the low-voltage (LV) regime (0.3V) with geometries from the 2019 and 2028 nodes of the 2013 International Technology Roadmap for Semiconductors (ITRS) are benchmarked along with an ultra-thin-body Si FET. Current can increase or decrease with scaling, and the trend is strongly correlated with the effective mass. For LV operation at the 2028 node, an effective mass of ~0.4 m0, corresponding to that of WSe2, gives the maximum drive current. The short 6 nm gate length combined with LV operation is forgiving in its requirements for material quality and contact resistances. In this LV regime, device and circuit performance are competitive using currently measured values for mobilities and contact resistances for the monolayer two-dimensional materials.",1611.06480v1 2016-12-28,In-plane anisotropy of transport coefficients in the electronic nematic states: Universal origin of the nematicity in Fe-based superconductors,"The origin of the electronic nematicity and its remarkable material-dependence are famous longstanding unsolved issues in Fe-based superconductors. To attack these issues, we focus on the in-plane anisotropy of the resistivity: In the nematic state in FeSe, the relation $\rho_x>\rho_y$ holds, where $\rho_{x(y)}$ is the resistivity along the longer (shorter) Fe-Fe axis. In contrast, the opposite anisotropy $\rho_x<\rho_y$ is realized in other undoped Fe-based superconductors. Such nontrivial material dependence is naturally explained in terms of the strongly orbital-dependent inelastic quasiparticle scattering realized in the orbital-ordered state. The opposite anisotropy between FeSe ($\rho_x>\rho_y$) and other undoped compounds ($\rho_x<\rho_y$) reflects the difference in the number of hole-pockets. We also explain the large in-plane anisotropy of the thermoelectric power in the nematic state.",1612.08841v1 2017-02-03,"Evolution of structure, magnetism and electronic transport in doped pyrochlore iridate Y$_2$Ir$_{2-x}$Ru$_{x}$O$_7$","The interplay between spin-orbit coupling (SOC) and electron correlation ($U$) is considered for many exotic phenomena in iridium oxides. We have investigated the evolution of structural, magnetic and electronic properties in pyrochlore iridate Y$_2$Ir$_{2-x}$Ru$_{x}$O$_7$ where the substitution of Ru has been aimed to tune this interplay. The Ru substitution does not introduce any structural phase transition, however, we do observe an evolution of lattice parameters with the doping level $x$. X-ray photoemission spectroscopy (XPS) study indicates Ru adopts charge state of Ru$^{4+}$ and replaces the Ir$^{4+}$ accordingly. Magnetization data reveal both the onset of magnetic irreversibility and the magnetic moment decreases with progressive substitution of Ru. These materials show non-equilibrium low temperature magnetic state as revealed by magnetic relaxation data. Interestingly, we find magnetic relaxation rate increases with substitution of Ru. The electrical resistivity shows an insulating behavior in whole temperature range, however, resistivity decreases with substitution of Ru. Nature of electronic conduction has been found to follow power-law behavior for all the materials.",1702.01023v1 2017-02-25,Compressive mechanical response of graphene foams and their thermal resistance with copper interfaces,"We report compressive mechanical response of graphene foams (GFs) and the thermal resistance ($R_{TIM}$) between copper (Cu) and GFs, where GFs were prepared by the chemical vapor deposition (CVD) method. We observe that Young's modulus ($E_{GF}$) and compressive strength ($\sigma_{GF}$) of GFs have a power law dependence on increasing density ($\rho_{GF}$) of GFs. The maximum efficiency of absorbed energy ($\eta_{max}$) for all GFs during the compression is larger than ~0.39. We also find that a GF with a higher $\rho_{GF}$ shows a larger $\eta_{max}$. In addition, we observe that the measured $R_{TIM}$ of Cu/GFs at room temperature with a contact pressure of 0.25 MP applied increases from ~50 to ~90 $mm^2K/W$ when $\rho_{GF}$ increases from 4.7 to 31.9 $mg/cm^3$.",1702.07816v1 2017-11-22,Structural properties of Fe/Cu magnetic multilayers: a Monte Carlo approach,"Using atomistic Monte Carlo simulations, we investigated the impact of the interface on the structural properties of iron and copper (Fe/Cu) magnetic multilayers grown by Vorono\""i diagram. Interest in magnetic multilayers has recently emerged as they are shown to be promising candidates for magnetic storage media, magneto-resistive sensors, and personalized medical treatment. As these artificial materials show large differences in properties compared to conventional ones, many experimental and theoretical works have been dedicated on shedding light on these differences and tremendous results have emerged. However, little is known how the interfaces influence the structure of the layers around them. By a numerical approach, we show that the structure of each layer depends on its thickness and the interface morphology. The Fe and Cu layers can adopt either the body-centered-cubic (bcc) or face-centered-cubic (fcc) structure, while the interface can assume amorphous, bcc, fcc, or a mixture of bcc and fcc structures depending on the layer thicknesses. These results are in good agreement with the experiments. They could be helpful in understanding effects such as giant magneto-resistance from the structural viewpoint.",1711.08508v1 2017-11-24,Inter-layer and Intra-layer Heat Transfer in Bilayer/Monolayer Graphene van der Waals Heterostructure: Is There a Kapitza Resistance Analogous?,"Van der Waals heterostructures have exhibited interesting physical properties. In this paper, heat transfer in hybrid coplanar bilayer/monolayer (BL-ML) graphene, as a model layered van der Waals heterostructure, was studied using non-equilibrium molecular dynamics (MD) simulations. Temperature profile and inter- and intra-layer heat fluxes of the BL-ML graphene indicated that, there is no fully developed thermal equilibrium between layers and the drop in average temperature profile at the step-like BL-ML interface is not attributable to the effect of Kapitza resistance. By increasing the length of the system up to 1 $\mu$m in the studied MD simulations, the thermally non-equilibrium region was reduced to a small area near the step-like interface. All MD results were compared to a continuum model and a good match was observed between the two approaches. Our results provide a useful understanding of heat transfer in nano- and micro-scale layered 2D materials and van der Waals heterostructures.",1711.09127v1 2018-04-20,Comparative study of the compensated semi-metals LaBi and LuBi : A first-principles approach,"We have investigated the electronic structures of LaBi and LuBi, employing the full-potential all electron method as implemented in Wien2k. Using this, we have studied in detail both the bulk and the surface states of these materials. From our band structure calculations we find that LuBi, like LaBi, is a compensated semi-metal with almost equal and sizable electron and hole pockets. In analogy with experimental evidence in LaBi, we thus predict that LuBi will also be a candidate for extremely large magneto-resistance (XMR), which should be of immense technological interest. Our calculations reveal that LaBi, despite being gapless in the bulk spectrum, displays the characteristic features of a $\mathbb{Z}_{2}$ topological semi-metal, resulting in gapless Dirac cones on the surface, whereas LuBi only shows avoided band inversion in the bulk and is thus a conventional compensated semi-metal with extremely large magneto-resistance.",1804.07652v1 2014-08-02,Destroyed quantum Hall effect in graphene with [0001] tilt grain boundaries,"The reason why the half-integer quantum Hall effect (QHE) is suppressed in graphene grown by chemical vapor deposition (CVD) is unclear. We propose that it might be connected to extended defects in the material and present results for the quantum Hall effect in graphene with [0001] tilt grain boundaries connecting opposite sides of Hall bar devices. Such grain boundaries contain 5-7 ring complexes that host defect states that hybridize to form bands with varying degree of metallicity depending on grain boundary defect density. In a magnetic field, edge states on opposite sides of the Hall bar can be connected by the defect states along the grain boundary. This destroys Hall resistance quantization and leads to non-zero longitudinal resistance. Anderson disorder can partly recover quantization, where current instead flows along returning paths along the grain boundary depending on defect density in the grain boundary and on disorder strength. Since grain sizes in graphene made by chemical vapor deposition are usually small, this may help explain why the quantum Hall effect is usually poorly developed in devices made of this material.",1408.0394v1 2019-02-21,Correlation in transport coefficients of hole-doped CuRhO$_2$ single crystals,"To clarify the origin of the nontrivial thermoelectric properties observed in the delafossite oxide CuRhO$_2$ polycrystals, we have performed the systematic transport measurements on the single-crystalline CuRhO$_2$ samples. In the parent compound, we find a pronounced peak structure due to a phonon-drag effect in the temperature dependence of the Seebeck coefficient, which is also confirmed by the size effect experiments. In the Mg-substituted crystals, in contrast to the results of the polycrystals, both the resistivity and the Seebeck coefficient decrease with increasing Mg content $y$. In particular, the coefficient $A$ for the $T^2$ term of the resistivity and the $T$-linear coefficient for the Seebeck coefficient at low temperatures are well described within a simple relationship expected for metals, which is also applicable to the correlated materials with low carrier densities.",1902.08301v1 2020-04-14,Temperature overshoot as the cause of physical changes in resistive switching devices during electro-formation,"Resistive switching devices based on transition metal oxides require formation of a conductive filament in order for the device to be able to switch. Such filaments have been proposed to form by the reduction of the oxide due to application of the electric field, but this report seeks to rebut that interpretation. Frequently reported physical changes during electro-formation include delamination of electrodes, crystallization of functional oxide, intermixing of electrode and oxide materials, and extensive loss of oxygen presumably to the ambient. Here we show that most of these effects are not inherent to the formation and switching processes and instead are due to an experimental artifact: the discharge of parasitic capacitances in the forming circuit. Discharge of typical BNC cables can raise the temperature of the filament to between 2,000 and 5,000 K resulting in extensive physical changes. Discharge and associated effects mentioned above can be eliminated using an on-chip load element without affecting the ability to switch.",2004.06571v1 2020-09-04,Effective Thermal Conductivity of SrBi$_4$Ti$_4$O$_{15}$-La$_{0.7}$Sr$_{0.3}$MnO$_3$ Oxide composite: Role of Particle Size and Interface Thermal Resistance,"We present a novel approach to reduce the thermal conductivity ($\kappa$) in thermoelectric composite materials using acoustic impedance mismatch and the Debye model. Also, the correlation between interface thermal resistance (R$_{int}$) and the particle size of the dispersed phase on the k of the composite is discussed. In particular, the $\kappa$ of an oxide composite which consists of a natural superlattice Aurivillius phase (SrBi$_4$Ti$_4$O$_{15}$) as a matrix and perovskite (La$_{0.7}$Sr$_{0.3}$MnO$_3$) as a dispersed phase is investigated. A significant reduction in the $\kappa$ of composite, even lower than the $\kappa$ of the matrix when the particle size of La$_{0.7}$Sr$_{0.3}$MnO$_3$ is smaller than the Kapitza radius (a$_K$) is observed, depicting that R$_{int}$ dominates for particle size lower than a$_K$ due to increased surface to volume ratio. The obtained results have the potential to provide new directions for engineering composite thermoelectric systems with desired thermal conductivity and promising in the field of energy harvesting.",2009.02218v1 2022-02-25,Low-Temperature Thermal Conductivity of CeRh$_{2}$As$_{2}$,"CeRh$_2$As$_2$ is a rare unconventional superconductor ($T_c=0.26$ K) characterized by two adjacent superconducting phases for a magnetic field $H \parallel c$-axis of the tetragonal crystal structure. Antiferromagnetic order, quadrupole-density-wave order ($T_0 = 0.4$ K) and the proximity of this material to a quantum-critical point have also been reported: The coexistence of these phenomena with superconductivity is currently under discussion. Here, we present thermal conductivity and electrical resistivity measurements on a single crystal of CeRh$_2$As$_2$ between 60 mK and 200 K and in magnetic fields ($H \parallel c$) up to 8 T. Our measurements at low $T$ verify the Wiedemann-Franz law within the error bars. The $T$ dependence of the thermal conductivity $\kappa(T)$ shows a pronounced drop below $T_c$ which is also field dependent and thus interpreted as the signature of superconductivity. However, the large residual resistivity and the lack of sharp anomalies in $\kappa(T)$ at the expected transition temperatures clearly indicate that samples of much higher purity are required to gain more information about the superconducting gap structure.",2202.12667v1 2016-03-07,Pressure-resistant intermediate valence in Kondo insulator SmB6,"Resonant x-ray emission spectroscopy (RXES) was used to determine the pressure dependence of the f-electron occupancy in the Kondo insulator SmB6. Applied pressure reduces the f-occupancy, but surprisingly, the material maintains a significant divalent character up to a pressure of at least 35 GPa. Thus, the closure of the resistive activation energy gap and onset of magnetic order are not driven by stabilization of an integer valent state. Over the entire pressure range, the material maintains a remarkably stable intermediate valence that can in principle support a nontrivial band structure.",1603.02207v1 2017-04-01,Small-signal model for 2D-material based field-effect transistors targeting radio-frequency applications: the importance of considering non-reciprocal capacitances,"A small-signal equivalent circuit of 2D-material based field-effect transistors is presented. Charge conservation and non-reciprocal capacitances have been assumed so the model can be used to make reliable predictions at both device and circuit levels. In this context, explicit and exact analytical expressions of the main radio-frequency figures of merit of these devices are given. Moreover, a direct parameter extraction methodology is provided based on S-parameter measurements. In addition to the intrinsic capacitances, transconductance and output conductance, our approach allows extracting the series combination of drain/source metal contact and access resistances. Accounting for these extrinsic resistances is of upmost importance when dealing with low dimensional field-effect transistors.",1704.00181v2 2017-04-05,An open-source platform to study uniaxial stress effects on nanoscale devices,"We present an automatic measurement platform that enables the characterization of nanodevices by electrical transport and optical spectroscopy as a function of uniaxial stress. We provide insights into and detailed descriptions of the mechanical device, the substrate design and fabrication, and the instrument control software, which is provided under open-source license. The capability of the platform is demonstrated by characterizing the piezo-resistance of an InAs nanowire device using a combination of electrical transport and Raman spectroscopy. The advantages of this measurement platform are highlighted by comparison with state-of-the-art piezo-resistance measurements in InAs nanowires. We envision that the systematic application of this methodology will provide new insights into the physics of nanoscale devices and novel materials for electronics, and thus contribute to the assessment of the potential of strain as a technology booster for nanoscale electronics.",1704.01394v1 2017-08-09,Contact-Induced Semiconductor-to-Metal Transition in Single-Layer WS$_2$,"Low-resistance ohmic contacts are a challenge for electronic devices based on two-dimensional materials. We show that an atomically precise junction between a two-dimensional semiconductor and a metallic contact can lead to a semiconductor-to-metal transition in the two-dimensional material--a finding which points the way to a possible method of achieving low-resistance junctions. Specifically, single-layer WS$_2$ undergoes a semiconductor-to-metal transition when epitaxially grown on Ag(111), while it remains a direct band gap semiconductor on Au(111). The metallicity of the single layer on Ag(111) is established by lineshape analysis of core level photoemission spectra. Angle-resolved photoemission spectroscopy locates the metallic states near the Q point of the WS$_2$ Brillouin zone. Density functional theory calculations show that the metallic states arise from hybridization between Ag bulk bands and the local conduction band minimum of WS$_2$ near the Q point.",1708.02799v1 2019-08-26,Local electrodynamics of a disordered conductor model system measured with a microwave impedance microscope,"We study the electrodynamic impedance of percolating conductors with a pre-defined network topology using a scanning microwave impedance microscope (sMIM) at GHz frequencies. For a given percolation number we observe strong spatial variations across a sample which correlate with the connected regions (clusters) in the network when the resistivity is low such as in Aluminum. For the more resistive material NbTiN the impedance becomes dominated by the local structure of the percolating network (connectivity). The results can qualitatively be understood and reproduced with a network current spreading model based on the pseudo-inverse Laplacian of the underlying network graph.",1908.09810v1 2019-11-30,Structural relaxation in amorphous materials under cyclic tension-compression loading,"The process of structural relaxation in disordered solids subjected to repeated tension-compression loading is studied using molecular dynamics simulations. The binary glass is prepared by rapid cooling well below the glass transition temperature and then periodically strained at constant volume. We find that the amorphous system is relocated to progressively lower potential energy states during hundreds of cycles, and the energy levels become deeper upon approaching critical strain amplitude from below. The decrease in potential energy is associated with collective nonaffine rearrangements of atoms, and their rescaled probability distribution becomes independent of the cycle number at sufficiently large time intervals. It is also shown that yielding during startup shear deformation occurs at larger values of the stress overshoot in samples that were cyclically loaded at higher strain amplitudes. These results might be useful for mechanical processing of amorphous alloys in order to reduce their energy and increase chemical resistivity and resistance to crystallization.",1912.00221v1 2021-01-04,Twin Mechanical Metamaterials,"By mimicking the geometrical relation of nano-twin crystals, we propose novel architected twin mechanical metamaterials (TMMs), which can impede local shearing band formation under external loading, thus avoiding global catastrophic failure. The effects of twin-space and twin angle on the mechanical performance of TMMs were also explored, such as: energy absorption, strength, and crack propagation resistance. The results showed that the twin topology design can not only significantly improve the energy-absorption efficiency but also remarkably improve the crack-propagation resistances of stretching-dominant mechanical metamaterials. We also studied the effect of twin-space and twin angle on the tensile strength of TMMs. This study is the first to report on the inverse Hall-Petch effect of TMMs. Our findings open an avenue for the design and fabrication of advanced materials with exceptionally tuneable mechanical properties.",2101.00927v1 2012-06-04,Optimal Condition for Strong Terahertz Radiation from Intrinsic Josephson Junctions,"In order to enhance the radiation power in terahertz band based on the intrinsic Josephson junctions of Bi$_2$Sr$_2$CaCu$_2$O$_{8+\delta}$ single crystal, we investigate a long cylindrical sample embedded in a dielectric material. Tuning the dielectric constant, the radiation power has a maximum which is achieved when it equals the dissipation caused by Josephson plasma. This yields the optimal dielectric constant of wrapping material in terms of the properties of BSCCO single crystal. The maximal radiation power is found proportional to the product of the typical superconducting current squared and the typical normal resistance, or the gap energy squared divided by the typical normal resistance, which offers a guideline for choosing superconductor as a source of strong radiation. By introducing an anti-reflection layer, we can build a compact device with the BSCCO cylinder and two wrapping dielectric layers with finite thicknesses.",1206.0516v1 2012-06-15,Breakdown of the interlayer coherence in twisted bilayer graphene,"Coherent motion of the electrons in the Bloch states is one of the fundamental concepts of the charge conduction in solid state physics. In layered materials, however, such a condition often breaks down for the interlayer conduction, when the interlayer coupling is significantly reduced by e.g. large interlayer separation. We report that complete suppression of coherent conduction is realized even in an atomic length scale of layer separation in twisted bilayer graphene. The interlayer resistivity of twisted bilayer graphene is much higher than the c-axis resistivity of Bernal-stacked graphite, and exhibits strong dependence on temperature as well as on external electric fields. These results suggest that the graphene layers are significantly decoupled by rotation and incoherent conduction is a main transport channel between the layers of twisted bilayer graphene.",1206.3410v1 2015-07-23,"Electronic, magnetic and transport properties of Fe intercalated 2H-TaS$_2$ studied by means of the KKR-CPA method","The electronic, magnetic and transport properties of Fe intercalated 2H-TaS$_2$ have been investigated by means of the Korringa-Kohn-Rostoker (KKR) method. The non-stoichiometry and disorder in the system has been accounted for using the Coherent Potential Approximation (CPA) alloy theory. A pronounced influence of disorder on the spin magnetic moment has been found for the ferro-magnetically ordered material. The same applies for the spin-orbit induced orbital magnetic moment and magneto-crystalline anisotropy energy. The temperature-dependence of the resistivity of disordered 2H-Fe$_{0.28}$TaS$_2$ investigated on the basis of the Kubo-St\v{r}eda formalism in combination with the alloy analogy model has been found in very satisfying agreement with experimental data. This also holds for the temperature dependent anomalous Hall resistivity $ \rho_{\rm xy}(T) $. The role of thermally induced lattice vibrations and spin fluctuations for the transport properties is discussed in detail.",1507.06544v1 2018-07-18,Thermoelectric stack sample cooling modification of a commercial atomic force microscopy,"Enabling temperature dependent experiments in Atomic Force Microscopy is of great interest to study materials and surface properties at the nanoscale. By studying Curie temperature of multiferroic materials, temperature based phase transition on crystalline structures or resistive switching phenomena are only a few examples of applications. We present an equipment capable of cooling samples using a thermoelectric cooling stage down to -61.4 C in a 15x15 mm sample plate. The equipment uses a four-unit thermoelectric stack to achieve maximum temperature range, with low electrical and mechanical noise. The equipment is installed into a Keysight 5500LS Atomic Force Microscopy maintaining its compatibility with all Electrical and Mechanical modes of operation. We study the contribution of the liquid cooling pump vibration into the cantilever static deflection noise and the temperature dependence of the cantilever deflection. A La0.7Sr0.3MnO3-y thin film sample is used to demonstrate the performance of the equipment and its usability by analysing the resistive switching phenomena associated with this oxide perovskite.",1807.06876v1 2019-01-21,Ferromagnetic Kondo lattice behavior in Ce11Pd4In9,"We report on the low-temperature physical properties of a novel compound Ce$_{11}$Pd$_4$In$_9$ that crystallizes with the orthorhombic Nd$_{11}$Pd$_4$In$_9$-type crystal structure (space group $Cmmm$). The compound exhibits ferromagnetic ordering at $T_{\rm {C}}$ = 18.6 K and an order-order transition at $T_{\rm {t}}$ $\sim$~1.6 K, as inferred from the low-temperature magnetic susceptibility, heat capacity and electrical resistivity data. In the paramagnetic region, the electrical transport in Ce$_{11}$Pd$_4$In$_9$ is dominated by Kondo effect. Below $T_{\rm {C}}$, a distinct contribution due to ferromagnetic spin waves dominates the electrical resistivity data, while at the lowest temperatures, the electrical transport and thermodynamic properties are governed by strong electron-electron correlations. The features observed conjointly hint at strongly correlated ground state in Ce$_{11}$Pd$_4$In$_9$ .",1901.06888v1 2019-11-14,Absence of evidence of spin transport through amorphous Y$_3$Fe$_5$O$_{12}$,"Long-distance transport of spin information in insulators without long-range magnetic order has been recently reported. Here, we perform a complete characterization of amorphous Y$_3$Fe$_5$O$_{12}$ (a-YIG) films grown on top of SiO$_2$. We confirm a clear amorphous structure and paramagnetic behavior of our a-YIG films, with semiconducting behavior resistivity that strongly decays with increasing temperature. The non-local transport measurements show a signal which is not compatible with spin transport and can be attributed to the drop of the a-YIG resistivity caused by Joule heating. Our results emphasize that exploring spin transport in amorphous materials requires careful procedures in order to exclude the charge contribution from the spin transport signals.",1911.06061v2 2019-11-15,Design and Performance of Hafnium Optical and Near-IR Kinetic Inductance Detectors,"We report on the design and performance of Microwave Kinetic Inductance Detectors (MKIDs) sensitive to single photons in the optical to near-infrared range using hafnium as the sensor material. Our test device had a superconducting transition temperature of 395 mK and a room temperature normal state resistivity of 97 $\mu \Omega$ cm with an RRR = 1.6. Resonators on the device displayed internal quality factors of around 200,000. Similar to the analysis of MKIDs made from other highly resistive superconductors, we find that modeling the temperature response of the detector requires an extra broadening parameter in the superconducting density of states. Finally, we show that this material and design is compatible with a full-array fabrication process which resulted in pixels with decay times of about 40 $\mu$s and resolving powers of ~9 at 800 nm.",1911.06434v1 2020-01-08,Effect of memory electrical switching in metal/vanadium oxide/silicon structures with VO2 films obtained by the sol-gel method,"Electrical switching and rectifying properties of the metal-VO2-Si structures, on both p-type and n-type silicon, with vanadium dioxide films obtained by an acetylacetonate sol-gel method, are studied. The switching effect is shown to be due to the semiconductor-to-metal phase transition (SMPT) in vanadium dioxide. The shift of the switching threshold voltage, accompanied by the memory effect, in forward bias of the p-Si-VO2 anisotype heterojunction is observed. To explain this effect, a model is proposed which suggests the existence of an additional series resistance associated with a channel at the VO2/Si interface, where a SiOx layer forms during the VO2 deposition process. This resistance is responsible for both threshold switching characteristics, and the memory effect, and the oxygen ion electromigration process is shown to underlie this effect. Potential applications of the observed phenomena, combining the effects of ReRAM and SMPT, in oxide electronics are discussed.",2001.03055v1 2020-05-24,"Schottky barriers, emission regimes and contact resistances in 2H-1T' MoS$_2$ lateral metal-semiconductor junctions from first-principles","We have studied the finite bias transport properties of a 2H-1T' MoS$_2$ lateral metal-semiconductor (M-S) junction by non-equilibrium Green's functions calculations, aimed at contacting the 2D channel in a field effect transistor. Our results indicate that (a) despite the fundamentally different electrostatics of line and planar dipoles, the Schottky barrier heights respond similarly to changes in doping and applied bias in 2D and 3D M-S junctions, (b) 2H-1T' MoS$_2$ lateral junctions are free from Fermi level pinning, (c) armchair interfaces have superior contacting properties vs.\ zigzag interfaces, (d) 1T' contacts to $p$ channels will present a reduced contact resistance by a factor of 4-10 with respect to $n$ channels and (e) contacts to intermediately doped $n$ ($p$) channels operate in the field (thermionic) emission regime. We also provide an improved procedure to experimentally determine the emission regime in 2D material junctions.",2005.11717v1 2020-06-12,Blocking of conducting channels widens window for ferroelectric resistive switching in interface-engineered Hf0.5Zr0.5O2 tunnel devices,"Films of Hf0.5Z0.5O2 (HZO) contain a network of grain boundaries. In (111) HZO epitaxial films on (001) SrTiO3, for instance, twinned orthorhombic (o-HZO) ferroelectric crystallites coexist with grain boundaries between o-HZO and a residual paraelectric monoclinic (m-HZO) phase. These grain boundaries contribute to the resistive switching response in addition to the genuine ferroelectric polarization switching and have detrimental effects on device performance. Here, it is shown that, by using suitable nanometric capping layers deposited on HZO film, a radical improvement of the operation window of the tunnel device can be achieved. Crystalline SrTiO3 and amorphous AlOx are explored as capping layers. It is observed that these layers conformally coat the HZO surface and allow to increase the yield and homogeneity of functioning ferroelectric junctions while strengthening endurance. Data show that the capping layers block ionic-like transport channels across grain boundaries. It is suggested that they act as oxygen suppliers to the oxygen-getters grain boundaries in HZO. In this scenario it could be envisaged that these and other oxides could also be explored and tested for fully compatible CMOS technologies.",2006.07048v1 2020-07-09,Fe3Se4: A Possible Ferrimagnetic Half-Metal?,"Half-metallic ferromagnets show 100% spin-polarization at the Fermi level and are ideal candidates for spintronic applications. Despite the extensive research in the field, very few materials have been discovered so far. Here we present results of electronic band structure calculations based on density functional theory and extensive physical-property measurements for Fe3Se4 revealing signatures of half-metallicity. The spin-polarized electronic band structure calculations predict half-metallic ferrimagnetism for Fe3Se4. The electrical resistivity follows exponentially suppressed electron-magnon scattering mechanism in the low-temperature regime and show a magnetoresistance effect that changes the sign from negative to positive with decreasing temperature around 100 K. Other intriguing observations include the anomalous behavior of Hall resistance below 100 K and an anomalous Hall coefficient that roughly follows the \r{ho}2 behavior.",2007.04736v1 2020-07-29,Quasiparticle and Nonquasiparticle Transport in Doped Quantum Paraelectrics,"Charge transport in doped quantum paralectrics (QPs) presents a number of puzzles, including a pronounced $T^2$ regime in the resistivity. We analyze charge transport in a QP within a model of electrons coupled to a soft transverse optical (TO) mode via a two-phonon mechanism. For $T$ above the soft-mode frequency but below some characteristic scale ($E_0$), the resistivity scales with the occupation number of phonons squared, i.e., as $T^2$. The $T^2$ scattering rate does not depend on the carrier number density and is not affected by a crossover between degenerate and non-degenerate regimes, in agreement with the experiment. Temperatures higher than $E_0$ correspond to a non-quasiparticle regime, which we analyze by mapping the Dyson equation onto a problem of supersymmetric quantum mechanics. The combination of scattering by two TO phonons and by a longitudinal optical mode explains the data quite well.",2007.14947v2 2020-08-06,"Magnetic, transport, and thermal properties of $δ$-phase UZr$_2$","Alloys of hexagonal $\delta$-phase UZr$_2$ have been synthesized and studied by means of heat capacity, magnetic susceptibility, magnetization, electrical resistivity, magnetoresistance, thermoelectric power, thermal conductivity measurements, for the first time, at temperatures from 1.8 to 300 K and in magnetic fields up to 8 T. The weak temperature dependence of the magnetic susceptibility and the small value of both Seebeck (0.75 $\mu$V/K at room temperature) and of the Sommerfeld coefficient (13.5 mJ mol$^{-1}$ K$^{-2}$) point to 5$f$-electrons in this material having a delocalized nature. The electrical resistivity and magnetoresistance indicate the presence of significant electronic disorder in $\delta$-UZr$_2$, consistent with the disorder in its crystal structure. Density functional theory calculations have been performed and compared to experimental results.",2008.02746v1 2020-12-29,Magnetotransport signatures of chiral magnetic anomaly in the half-Heusler phase ScPtBi,"Study of magnetotransport properties of ScPtBi revealed simultaneously: a negative contribution to the longitudinal magnetoresistance, the planar Hall effect, and distinct angular narrowing of the longitudinal magnetoresistance { three hallmarks of chiral magnetic anomaly (pumping of axial charge between Weyl nodes), a distinct property of topological semimetals. Electronic structure calculations show that structural defects, such as antisites and vacancies, bring substantial density of states at the Fermi level of ScPtBi, indicating that it is a semimetal, not a zero-gap semiconductor, as predicted earlier. This is in accord with electrical resistivity in ScPtBi, showing no characteristics of semiconductor. Moreover, below 0.7K we observed an onset of a superconducting transition, with the resistivity disappearing completely below 0.23 K.",2012.14819v2 2021-05-28,Projected mushroom-type phase-change memory,"Phase-change memory devices have found applications in in-memory computing where the physical attributes of these devices are exploited to compute in place without the need to shuttle data between memory and processing units. However, non-idealities such as temporal variations in the electrical resistance have a detrimental impact on the achievable computational precision. To address this, a promising approach is projecting the phase configuration of phase change material onto some stable element within the device. Here we investigate the projection mechanism in a prominent phase-change memory device architecture, namely mushroom-type phase-change memory. Using nanoscale projected Ge2Sb2Te5 devices we study the key attributes of state-dependent resistance, drift coefficients, and phase configurations, and using them reveal how these devices fundamentally work.",2105.13693v2 2021-08-04,Current-induced breakdown of the quantum anomalous Hall effect,"The quantum anomalous Hall effect (QAHE) realizes dissipationless longitudinal resistivity and quantized Hall resistance without the need of an external magnetic field. However, when reducing the device dimensions or increasing the current density, an abrupt breakdown of the dissipationless state occurs with a relatively small critical current, limiting the applications of the QAHE. We investigate the mechanism of this breakdown by studying multi-terminal devices and identified that the electric field created between opposing chiral edge states lies at the origin. We propose that electric-field-driven percolation of two-dimensional charge puddles in the gapped surface states of compensated topological-insulator films is the most likely cause of the breakdown.",2108.02081v1 2021-10-08,Universal Non-Volatile Resistive Switching Behavior in 2D Metal Dichalcogenides Featuring Unique Conductive-Point Random Access Memory Effect,"Two-dimensional materials have been discovered to exhibit non-volatile resistive switching (NVRS) phenomenon. In our work, we reported the universal NVRS behavior in a dozen metal dichalcogenides, featuring low switching voltage, large on/off ratio, fast switching speed and forming free characteristics. A unique conductive-point random access memory (CPRAM) effect is used to explain the switching mechanisms, supported by experimental results from current-sweep measurements.",2110.03863v1 2021-10-27,Bound on resistivity in flat-band materials due to the quantum metric,"The quantum metric is a central quantity of band theory but has so far not been related to many response coefficients due to its nonclassical origin. However, within a newly developed Kubo formalism for fast relaxation, the decomposition of the dc electrical conductivity into both classical (intraband) and quantum (interband) contributions recently revealed that the interband part is proportional to the quantum metric. Here, we show that interband effects due to the quantum metric can be significantly enhanced and even dominate the conductivity for semimetals at charge neutrality and for systems with highly quenched bandwidth. This is true in particular for topological flat-band materials of nonzero Chern number, where for intermediate relaxation rates an upper bound exists for the resistivity due to the common geometrical origin of quantum metric and Berry curvature. We suggest to search for these effects in highly tunable rhombohedral trilayer graphene flakes.",2110.14658v3 2021-11-22,First-principles-based screening method for resistivity scaling of anisotropic metals,"The resistivity scaling of metals is a crucial limiting factor for further downscaling of interconnects in nanoelectronic devices that affects signal delay, heat production, and energy consumption. Here, we generalize a commonly considered figure of merit for selecting promising candidate metals with highly anisotropic Fermi surfaces in terms of their electronic transport properties at the nanoscale. For this, we introduce a finite-temperature transport tensor, based on band structures obtained from first principles. This transport tensor allows for a straightforward comparison between highly anisotropic metals in nanostructures with different lattice orientations and arbitrary transport directions. By evaluating the temperature dependence of the tensor components, we also assess the validity of a Fermi surface-based evaluation of the transport properties at zero temperature, rather than considering standard operating temperature conditions.",2111.11121v2 2021-12-17,Nanoscale laser flash measurements of diffuson transport in amorphous Ge and Si,"The thermal properties of amorphous materials have attracted significant attention due to their technological importance in electronic devices. Additionally, the disorder-induced breakdown of the phonon gas model makes vibrational transport in amorphous materials a topic of fundamental interest. In the past few decades, theoretical concepts such as propagons, diffusons, and locons have emerged to describe different types of vibrational modes in disordered solids. But experiments can struggle to accurately determine which types of vibrational states carry the majority of the heat. In the present study, we use nanoscale laser flash measurements (front/back time-domain thermoreflectance) to investigate thermal transport mechanisms in amorphous Ge and amorphous Si thin-films. We observe a nearly linear relationship between the amorphous film's thermal resistance and the film's thickness. The slope of the film's thermal resistance vs. thickness corresponds to a thickness-independent thermal conductivity of 0.4 and 0.6 W/(m-K) for a-Ge and a-Si, respectively. This result reveals that the majority of heat currents in amorphous Si and Ge thin films prepared via RF sputtering at room temperature are carried by diffusons and/or propagons with mean free paths less than a few nanometers.",2112.09289v2 2022-01-06,Insights to negative differential resistance in \texorpdfstring{MoS\textsubscript{2}}{MoS2} Esaki diodes: a first-principles perspective,"\ce{MoS_2} is a two dimensional material with a band gap depending on the number of layers and tunable by an external electric field. The experimentally observed intralayer band-to-band tunneling and interlayer band-to-band tunneling in this material present an opportunity for new electronic applications in tunnel field effect transistors. However, such a widely accepted concept has never been supported up by theoretical investigations based on first principles. In this work, using density functional theory, in conjunction with non-equilibrilibrium Green's function techniques and our electric field gating method, enabled by a large-scale computational approach, we study the relation between band alignment and transmission in planar and side-stack \ce{MoS_2} $p$-$i$-$n$ junction configurations. We demonstrate the presence of negative differential resistance for both in-plane and interlayer current, a staple characteristic of tunnel diode junctions, and analyze the physical origin of such an effect. Electrostatic potentials, the van der Waals barrier, and complex band analysis are also examined for a thorough understanding of Esaki Diodes.",2201.02178v1 2022-05-21,Increased Phase Coherence Length in a Porous Topological Insulator,"The surface area of Bi2Te3 thin films was increased by introducing nanoscale porosity. Temperature dependent resistivity and magnetotransport measurements were conducted both on as-grown and porous samples (23 and 70 nm). The longitudinal resistivity of the porous samples became more metallic, indicating the increased surface area resulted in transport that was more surface-like. Weak antilocalization (WAL) was present in all samples, and remarkably the phase coherence length doubled in the porous samples. This increase is likely due to the large Fermi velocity of the Dirac surface states. Our results show that the introduction of nanoporosity does not destroy the topological surface states but rather enhances them, making these nanostructured materials promising for low energy electronics, spintronics and thermoelectrics.",2205.10589v1 2022-07-11,Spin-Orbit Proximity Effect in Bi/Co Multilayer: The Role of Interface Scattering,"The Spin-Orbit Proximity Effect is the raise of Spin-Orbit Coupling at a layer near to the interface with a strong spin-orbit material. It has been seen in several system such as graphene and ferromagnetic layers. The control of the Spin-Orbit Coupling can be a pathway to discover novel and exotic phases in superconductor and semimetallic systems. Here, we study the magnetoelectrical transport, i.e., magnetoresistance and anomalous Hall effect, in Cobalt/Bismuth multilayers looking for traces of spin-orbit proximity effect and evaluate the origin of such effect. Our results point for an increase of Spontaneous Magnetic Anisotropy of Resistivity and Anomalous Hall Resistivity at very low thicknesses of Cobalt. The analysis of the Anomalous Hall Resisitivity indicate that the Bismuth layers change the scattering mechanism of Hall effect to the extrinsic skew-scattering type, indicating that the spin-orbit proximity effect could be related to the elastic scattering of cobalt free carriers by bismuth sites at the interface.",2207.04937v1 2022-08-22,Unified intermediate coupling description of the pseudogap and the strange metal phases of cuprates,"A one band Hubbard model with intermediate coupling is shown to describe the two most important unusual features of a normal state: linear resistivity strange metal and the pseudogap. Both the spectroscopic and transport properties of the cuprates are considered on the same footing by employing a relatively simple postgaussian approximation valid for the intermediate couplings $U/t=1.5-4$ in relevant temperatures $T>100{\rm K}.$ In the doping range $\ p=0.1-0.3$, the value of $U$ is smaller than that in the parent material. For a smaller doping, especially in the Mott insulator phase, the coupling is large compared to the effective tight binding scale and a different method is required. This scenario provides an alternative to the paradigm that the coupling should be strong, say $U/t>6$, in order to describe the strange metal. We argue that to obtain phenomenologically acceptable underdoped normal state characteristics like $T^{\ast }$, pseudogap values, and spectral weight distribution, a large value of $U$ is detrimental. Surprisingly the resistivity in the above temperature range is linear $\rho =\rho_{0}+\alpha \frac{m^{\ast }}{e^{2}n\hbar }T$ with the ""Planckian"" coefficient $\alpha $ of order one.",2208.10093v1 2022-09-05,Charge-Density Wave Driven Giant Thermionic-Current Switching in 1T-TaS$_{2}$/2H-TaSe$_{2}$/2H-MoS$_{2}$ Heterostructure,"1T-TaS$_2$ exhibits several resistivity phases due to the modulation of charge density wave (CDW). The fact that such phase transition can be driven electrically has attracted a lot of attention in the recent past towards \emph{active-metal} based electronics. However, the bias-driven resistivity switching is not very large ($<$ 5 fold), and an enhancement in the same will highly impact such phase transition devices. One aspect that is often overlooked is that such phase transition is also accompanied by a significant change in the local temperature due to the low thermal conductivity of 1T-TaS$_2$. In this work, we exploit such electrically driven phase transition induced temperature change to promote carriers over a thermionic barrier in a 1T-TaS$_{2}$/2H-TaSe$_{2}$/2H-MoS$_{2}$ T-Junction, achieving a $964$-fold abrupt switching in the current through the MoS$_2$ channel. The device is highly reconfigurable and exhibits an abrupt reduction in current as well when the biasing configuration changes. The results are promising for several electronic applications, including neuromorphic chips, switching, nonlinear devices, and industrial electronics such as current and temperature sensing.",2209.02024v1 2022-11-18,Pressure-induced superconductivity in PdTeI with quasi-one-dimensional PdTe chains,"The quasi-one-dimensional material PdTeI exhibits unusual electronic transport properties at ambient pressure. Here, we systematically investigate both the structural and electronic responses of PdTeI to external pressure, through a combination of electrical transport, synchrotron x-ray diffraction (XRD), and Raman spectroscopy measurements. The charge density wave (CDW) order in PdTeI is fragile and the transition temperature TCDW decreases rapidly with the application of external pressure. The resistivity hump is indiscernible when the pressure is increased to 1 GPa. Upon further compression, zero resistance is established above 20 GPa, suggesting the occurrence of superconductivity. Combined XRD and Raman data evidence that the emergence of superconductivity is accompanied by a pressure-induced amorphization of PdTeI.",2211.10294v1 2023-02-21,Electron transport and scattering mechanisms in ferromagnetic monolayer Fe$_3$GeTe$_2$,"We study intrinsic charge-carrier scattering mechanisms and determine their contribution to the transport properties of the two-dimensional ferromagnet Fe$_3$GeTe$_2$. We use state-of-the-art first-principles calculations combined with the model approaches to elucidate the role of the electron-phonon and electron-magnon interactions in the electronic transport. Our findings show that the charge carrier scattering in Fe$_3$GeTe$_2$ is dominated by the electron-phonon interaction, while the role of magnetic excitations is marginal. At the same time, the magnetic ordering is shown to effect essentially on the electron-phonon coupling and its temperature dependence. This leads to a sublinear temperature dependence of the electrical resistivity near the Curie temperature, which is in line with experimental observations. The room temperature resistivity is estimated to be $\sim$35 $\mu \Omega \cdot$cm which may be considered as an intrinsic limit for monolayer Fe$_3$GeTe$_2$.",2302.10974v1 2023-03-20,Thermal decomposition of the Kitaev material $α$-RuCl$_3$ and its influence on low-temperature behavior,"We explore the effect of heat treatment in argon atmosphere under various temperatures up to $500^\circ$C on single crystals of $\alpha$-RuCl$_3$ by study of the mass loss, microprobe energy dispersive x-ray spectroscopy, powder x-ray diffraction, electrical resistance as well as low-temperature magnetic susceptibility and specific heat. Clear signatures of dechlorination and oxidation of Ru appear for annealing temperatures beyond $300^\circ$C. Analysis of the specific heat below 2~K reveals a RuO$_2$ mass fraction of order $1\%$ for pristine $\alpha$-RuCl$_3$ which increases up to $20\%$ after thermal annealing, fully consistent with mass-loss analysis. The small RuO$_2$ inclusions drastically reduce the global electrical resistance and may thus significantly affect low-temperature thermal transport and Hall effect.",2303.11308v1 2023-09-08,Re-entrance of resistivity due to the interplay of superconductivity and magnetism in $\ce{Eu_{0.73}Ca_{0.27}(Fe_{0.87}Co_{0.13})2As2}$,"By simultaneous Co and Ca-doping we were able to obtain an $\ce{EuFe2As2}$-based compound with superconductivity appearing above the antiferromagnetic order of $\ce{Eu^{2+}}$ magnetic moments. However, as soon as the antiferromagnetic order appears a re-entrance behavior is observed \textemdash{} instead of zero resistivity and diamagnetic signal down to the temperature of \unit[2]{K}. By investigating magnetization, ac susceptibility and electrical transport properties of $\ce{Eu_{0.73}Ca_{0.27}(Fe_{0.87}Co_{0.13})2As2}$ and comparing them to previously studied M\""ossbauer effect and neutron scattering measurements of this and similar compounds an explanation of such behavior is proposed.",2309.04308v2 2023-10-02,Crystallographic-dependent bilinear magnetoelectric resistance in a thin WTe$_2$ layer,"The recently reported Bilinear Magnetoeletric Resistance (BMR) in novel materials with rich spin textures, such as bismuth selenide (Bi$_2$Se$_3$) and tungsten ditelluride (WTe$_2$), opens new possibilities for probing the spin textures via magneto-transport measurements. By its nature, the BMR effect is directly linked to the crystal symmetry of the materials and its spin texture. Therefore, understanding the crystallographic dependency of the effect is crucial. Here we report the observation of crystallographic-dependent BMR in thin WTe$_2$ layers and explore how it is linked to its spin textures. The linear response measured in first harmonic signals and the BMR measured in second harmonic signals are both studied under a wide range of magnitudes and directions of magnetic field, applied current and at different temperatures. We discover a three-fold symmetry contribution of the BMR when current is applied along the a-axis of the WTe$_2$ thin layer at 10 K, which is absent for when current is applied along the b-axis.",2310.01058v1 2023-11-23,Helicoidal Transformation Method for Finite Element Models of Twisted Superconductors,"This paper deals with the modelling of superconducting and resistive wires with a helicoidal symmetry, subjected to an external field and a transport current. Helicoidal structures are three-dimensional, and therefore yield computationally intensive simulations in a Cartesian coordinate system. We show in this paper that by working instead with a helicoidal system of coordinates, the problem to solve can be made two-dimensional, drastically reducing the computational cost. We first introduce the state-of-the-art approach and apply it on the h-phi-formulation with helicoidally symmetric boundary conditions (e.g., axial external magnetic field, with or without transport current), with an emphasis on the function space discretization. Then, we extend the approach to general boundary conditions (e.g., transverse external magnetic field) and present numerical results with linear materials. In particular, we discuss the frequency-dependent losses in composite wires made of superconducting filaments embedded in a resistive matrix. Finally, we provide outlook to the application of the generalized model with nonlinear materials.",2311.13919v2 2024-03-28,"Single-Crystal Growth and Characterization of Cuprate Superconductor (Hg,Re)Ba$_2$Ca$_2$Cu$_3$O$_{8+δ}$","We grew (Hg,Re)Ba$_2$Ca$_2$Cu$_3$O$_{8+\delta}$ ((Hg,Re)1223) single crystals with good reproducibility via the single-step flux method using monoxides as raw materials. A double-sealing method using a thick-walled quartz tube and a stainless-steel container was adopted for explosion protection. The maximum crystal size was approximately 1 mm x 1 mm in the ab plane and 0.04 mm in thickness. The crystal was square-shaped, reflecting the tetragonal crystal structure of (Hg,Re)1223. Magnetic susceptibility measurements indicated a critical temperature of 130 K. The in-plane resistivity exhibited a linear temperature dependence, indicating that the sample was close to optimal doping level. The out-of-plane resistivity was also measured, and the anisotropy parameter was 250-650 at 300 K.",2403.19182v1 2024-05-01,Tunable viscous layers in Corbino geometry using density junctions,"In sufficiently clean materials where electron-electron interactions are strong compared to momentum-relaxing scattering processes, electron transport resembles the flow of a viscous fluid. We study hydrodynamic electron transport across density interfaces (n-n junctions) in a 2DEG in the Corbino geometry. From numerical simulations in COMSOL using realistic parameters, we show that we can produce tunable viscous layers at the density interface by varying the density ratio of charge carriers. We quantitatively explain this observation with simple analytic expressions together with boundary conditions at the interface. We also show signatures of these viscous layers in the magnetoresistance. Breaking down viscous and ohmic contributions, we find that when outer radial region of the Corbino has higher charge density compared to the inner region, the viscous layers at the interface serve to suppress the magneto-resistance produced by momentum-relaxing scattering. Conversely, the magneto-resistance is enhanced when the inner region has higher density than the outer. Our results add to the repertoire of techniques for engineering viscous electron flows, which hold a promise for applications in future electronic devices.",2405.00381v1 2003-06-06,Collective transport and optical absorption near the stripe criticality,"Within the stripe quantum critical point scenario for high $T_c$ superconductors, we point out the possible direct contribution of charge collective fluctuations to the optical absorption and to the d.c. resistivity.",0306176v1 2010-08-09,"Planes, Chains, and Orbits: Quantum Oscillations and High Magnetic Field Heat Capacity in Underdoped YBCO","The underlying physics of the magnetic-field-induced resistive state in high temperature cuprate superconductors remains a mystery. One interpretation is that the application of magnetic field destroys the d-wave superconducting gap to uncover a Fermi surface that behaves like a conventional (i.e.Fermi Liquid) metal (1). Another view is that an applied magnetic field destroys long range superconducting phase coherence, but the superconducting gap amplitude survives (2, 3). By measuring the specific heat of ultra-clean YBa2Cu3O6.56 (YBCO 6.56), we obtain a measure of the quasi-particle density of states from the superconducting state well into the magnetic-field-induced resistive state. We have found that at very high magnetic fields the specific heat exhibits both the conventional temperature dependence and quantum oscillations expected for a Fermi Liquid. On the other hand, the magnetic field dependence of the quasi-particle density of states follows a \sqrt{H} behavior that persists right through the zero-resistance transition, evidencing the fully developed d-wave superconducting gap over the entire magnetic field range measured. The coexistence of these two phenomena pose a rigorous thermodynamic constraint on theories of high-magnetic-field resistive state in the cuprates.",1008.1568v1 2011-02-09,Heavy Long-lived Mossbauer State of Niobium,"A heavy niobium state showing 1/3 residual resistance is discovered below the superconducting transition temperature. This niobium sample contains high-density long-lived Mossbauer excitation.",1102.1766v2 2015-12-21,"Kondo effect in CeX$_{c}$ (X$_{c}$=S, Se, Te) studied by electrical resistivity under high pressure","We have measured the electrical resistivity of cerium monochalcogenices, CeS, CeSe, and CeTe, under high pressures up to 8 GPa. Pressure dependences of the antiferromagnetic ordering temperature $T_{N}$, crystal field splitting, and the $\ln T$ anomaly of the Kondo effect have been studied to cover the whole region from the magnetic ordering regime at low pressure to the Fermi liquid regime at high pressure. $T_{N}$ initially increases with increasing pressure, and starts to decrease at high pressure as expected from the Doniach's diagram. Simultaneously, the $\ln T$ behavior in the resistivity is enhanced, indicating the enhancement of the Kondo effect by pressure. It is also characteristic in CeX$_{c}$ that the crystal field splitting rapidly decreases at a common rate of $-12.2$ K/GPa. This leads to the increase in the degeneracy of the $f$ state and further enhancement of the Kondo effect. It is shown that the pressure dependent degeneracy of the $f$ state is a key factor to understand the pressure dependence of $T_{N}$, Kondo effect, magnetoresistance, and the peak structure in the temperature dependence of resistivity.",1512.06530v1 2019-10-01,High transparency Bi2Se3 topological insulator nanoribbon Josephson junctions with low resistive noise properties,"Bi$_2$Se$_3$ nanoribbons, grown by catalyst-free Physical Vapour Deposition, have been used to fabricate high quality Josephson junctions with Al superconducting electrodes. The conductance spectra (dI/dV) of the junctions show clear dip-peak structures characteristic of multiple Andreev reflections. The temperature dependence of the dip-peak features reveals a highly transparent Al/Bi$_2$Se$_3$ topological insulator nanoribbon interface and Josephson junction barrier. This is supported by the high values of the Bi$_2$Se$_3$ induced gap and of I$_c$R$_n$ (I$_c$ critical current, R$_n$ normal resistance of the junction) product both of the order of 160 $\mu$eV, a value close to the Al gap. The devices present an extremely low relative resistance noise below 1$\times$10$^{-12}$ $\mu$m$^2$/Hz comparable to the best Al tunnel junctions, which indicates a high stability in the transmission coefficients of transport channels. The ideal Al/Bi$_2$Se$_3$ interface properties, perfect transparency for Cooper pair transport in conjunction with low resistive noise make these junctions a suitable platform for further studies of the induced topological superconductivity and Majorana bound states physics.",1910.00280v2 2017-04-28,Electric Field Effect in Multilayer Cr2Ge2Te6: a Ferromagnetic Two-Dimensional Material,"The emergence of two-dimensional (2D) materials has attracted a great deal of attention due to their fascinating physical properties and potential applications for future nanoelectronic devices. Since the first isolation of graphene, a Dirac material, a large family of new functional 2D materials have been discovered and characterized, including insulating 2D boron nitride, semiconducting 2D transition metal dichalcogenides and black phosphorus, and superconducting 2D bismuth strontium calcium copper oxide, molybdenum disulphide and niobium selenide, etc. Here, we report the identification of ferromagnetic thin flakes of Cr2Ge2Te6 (CGT) with thickness down to a few nanometers, which provides a very important piece to the van der Waals structures consisting of various 2D materials. We further demonstrate the giant modulation of the channel resistance of 2D CGT devices via electric field effect. Our results illustrate the gate voltage tunability of 2D CGT and the potential of CGT, a ferromagnetic 2D material, as a new functional quantum material for applications in future nanoelectronics and spintronics.",1704.08862v1 2023-09-26,"The p-Laplace ""Signature"" for Quasilinear Inverse Problems with Large Boundary Data","This paper is inspired by an imaging problem encountered in the framework of Electrical Resistance Tomography involving two different materials, one or both of which are nonlinear. Tomography with nonlinear materials is in the early stages of developments, although breakthroughs are expected in the not-too-distant future. We consider nonlinear constitutive relationships which, at a given point in the space, present a behaviour for large arguments that is described by monomials of order p and q. The original contribution this work makes is that the nonlinear problem can be approximated by a weighted p-Laplace problem. From the perspective of tomography, this is a significant result because it highlights the central role played by the $p-$Laplacian in inverse problems with nonlinear materials. Moreover, when p=2, this provides a powerful bridge to bring all the imaging methods and algorithms developed for linear materials into the arena of problems with nonlinear materials. The main result of this work is that for ""large"" Dirichlet data in the presence of two materials of different order (i) one material can be replaced by either a perfect electric conductor or a perfect electric insulator and (ii) the other material can be replaced by a material giving rise to a weighted p-Laplace problem.",2309.15206v1 2024-04-23,An Accessible Instrument for Measuring Soft Material Mechanical Properties,"Soft material research has seen significant growth in recent years, with emerging applications in robotics, electronics, and healthcare diagnostics where understanding material mechanical response is crucial for precision design. Traditional methods for measuring nonlinear mechanical properties of soft materials require specially sized samples that are extracted from their natural environment to be mounted on the testing instrument. This has been shown to compromise data accuracy and precision in various soft and biological materials. To overcome this, the Volume Controlled Cavity Expansion (VCCE) method was developed. This technique tests soft materials by controlling the formation rate of a liquid cavity inside the materials at the tip of an injection needle, and simultaneously measuring the resisting pressure which describes the material response. Despite VCCE's early successes, expansion of its application beyond academia has been hindered by cost, size, and expertise. In response to this, the first portable, bench-top instrument utilizing VCCE is presented here. This device, built with affordable, readily available components and open-source software, streamlines VCCE experimentation without sacrificing performance or precision. It is especially suitable for space-limited settings and designed for use by non-experts, promoting widespread adoption. The instrument's efficacy was demonstrated through testing Polydimethylsiloxane (PDMS) samples of varying stiffness. This study not only validates instrument performance, but also sets the stage for further advancements and broader applications in soft material testing. All data, along with acquisition, control, and post-processing scripts, are made available on GitHub.",2404.15036v1 2018-04-04,High-Performance Flexible Magnetic Tunnel Junctions for Smart Miniaturized Instruments,"Flexible electronics is an emerging field in many applications ranging from in vivo biomedical devices to wearable smart systems. The capability of conforming to curved surfaces opens the door to add electronic components to miniaturized instruments, where size and weight are critical parameters. Given their prevalence on the sensors market, flexible magnetic sensors play a major role in this progress. For many high-performance applications, magnetic tunnel junctions (MTJs) have become the first choice, due to their high sensitivity, low power consumption etc. MTJs are also promising candidates for non-volatile next-generation data storage media and, hence, could become central components of wearable electronic devices. In this work, a generic low-cost regenerative batch fabrication process is utilized to transform rigid MTJs on a 500 {\mu}m silicon wafer substrate into 5 {\mu}m thin, mechanically flexible silicon devices, and ensuring optimal utilization of the whole substrate. This method maintains the outstanding magnetic properties, which are only obtained by deposition of the MTJ on smooth high-quality silicon wafers. The flexible MTJs are highly reliable and resistive to mechanical stress. Bending of the MTJ stacks with a diameter as small as 500 {\mu}m is possible without compromising their performance and an endurance of over 1000 cycles without fatigue has been demonstrated. The flexible MTJs were mounted onto the tip of a cardiac catheter with 2 mm in diameter without compromising their performance. This enables the detection of magnetic fields and the angle which they are applied at with a high sensitivity of 4.93 %/Oe and a low power consumption of 0.15 {\mu}W, while adding only 8 {\mu}g and 15 {\mu}m to the weight and diameter of the catheter, respectively.",1804.01298v1 2017-01-30,High quality factor manganese-doped aluminum lumped-element kinetic inductance detectors sensitive to frequencies below 100 GHz,"Aluminum lumped-element kinetic inductance detectors (LEKIDs) sensitive to millimeter-wave photons have been shown to exhibit high quality factors, making them highly sensitive and multiplexable. The superconducting gap of aluminum limits aluminum LEKIDs to photon frequencies above 100 GHz. Manganese-doped aluminum (Al-Mn) has a tunable critical temperature and could therefore be an attractive material for LEKIDs sensitive to frequencies below 100 GHz if the internal quality factor remains sufficiently high when manganese is added to the film. To investigate, we measured some of the key properties of Al-Mn LEKIDs. A prototype eight-element LEKID array was fabricated using a 40 nm thick film of Al-Mn deposited on a 500 {\mu}m thick high-resistivity, float-zone silicon substrate. The manganese content was 900 ppm, the measured $T_c = 694\pm1$ mK, and the resonance frequencies were near 150 MHz. Using measurements of the forward scattering parameter $S_{21}$ at various bath temperatures between 65 and 250 mK, we determined that the Al-Mn LEKIDs we fabricated have internal quality factors greater than $2 \times 10^5$, which is high enough for millimeter-wave astrophysical observations. In the dark conditions under which these devices were measured, the fractional frequency noise spectrum shows a shallow slope that depends on bath temperature and probe tone amplitude, which could be two-level system noise. The anticipated white photon noise should dominate this level of low-frequency noise when the detectors are illuminated with millimeter-waves in future measurements. The LEKIDs responded to light pulses from a 1550 nm light-emitting diode, and we used these light pulses to determine that the quasiparticle lifetime is 60 {\mu}s.",1701.08461v2 1997-08-21,Charge Dynamics from Copper Oxide Materials,"The charge dynamics of the copper oxide materials in the underdoped and optimal doped regimes is studied within the framework of the fermion-spin theory. The conductivity spectrum shows the non-Drude behavior at low energies and unusual midinfrared peak, and the resistivity exhibits a linear behavior in the temperature, which are consistent with experiments and numerical simulations.",9708165v2 2000-07-06,Scaling of Crack Surfaces and Implications on Fracture Mechanics,"The scaling laws describing the roughness development of crack surfaces are incorporated into the Griffith criterion. We show that, in the case of a Family-Vicsek scaling, the energy balance leads to a purely elastic brittle behavior. On the contrary, it appears that an anomalous scaling reflects a R-curve behavior associated to a size effect of the critical resistance to crack growth in agreement with the fracture process of heterogeneous brittle materials exhibiting a microcracking damage.",0007100v1 2001-01-17,Negative Magnetoresistance Produced by Hall Fluctuations in a Ferromagnetic Domain Structure,"We present a model for a negative magnetoresistance (MR) that would develop in a material with many ferromagnetic domains even if the individual domains have no magnetoresistance and even if there is no boundary resistance. The negative MR is due to a classical current-distortion effect arising from spatial variations in the Hall conductivity, combined with a change in domain structure due to an applied magnetic field. The negative MR can exceed 1000% if the product of the carrier relaxation time and the internal magnetic field due to spontaneous magnetization is sufficiently large.",0101268v2 2001-03-06,Rheology of a confined granular material,"We study the rheology of a granular material slowly driven in a confined geometry. The motion is characterized by a steady sliding with a resistance force increasing with the driving velocity and the surrounding relative humidity. For lower driving velocities a transition to stick-slip motion occurs, exhibiting a blocking enhancement whith decreasing velocity. We propose a model to explain this behavior pointing out the leading role of friction properties between the grains and the container's boundary.",0103143v1 2001-11-07,Crumpling a Thin Sheet,"Crumpled sheets have a surprisingly large resistance to further compression. We have studied the crumpling of thin sheets of Mylar under different loading conditions. When placed under a fixed compressive force, the size of a crumpled material decreases logarithmically in time for periods up to three weeks. We also find hysteretic behavior when measuring the compression as a function of applied force. By using a pre-treating protocol, we control this hysteresis and find reproducible scaling behavior for the size of the crumpled material as a function of the applied force.",0111095v1 2003-10-23,Correlation between the Extraordinary Hall Effect and Resistivity,"We study the contribution of different types of scattering sources to the extraordinary Hall effect. Scattering by magnetic nano-particles embedded in normal-metal matrix, insulating impurities in magnetic matrix, surface scattering and temperature dependent scattering are experimentally tested. Our new data, as well as previously published results on a variety of materials, are fairly interpreted by a simple modification of the skew scattering model.",0310551v1 2003-12-29,La0.95Sr0.05CoO3: An efficient room-temperature thermoelectric oxide,"We present measurements of electrical resistivity, thermal conductivity and thermopower of polycrystalline Sr-doped LaCoO3 with composition La0.95Sr0.05CoO3. Our data show that the investigated compound exhibits a very respectable room temperature thermoelectric figure of merit value of 0.18. Our results not only show that oxides are promising candidates for thermoelectric cooling applications, but also point towards the need for careful theoretical calculations that will serve as a guide in producing the next generation of thermoelectric materials.",0312670v1 2004-01-06,"Superstructure, sodium ordering and antiferromagnetism in NaxCoO2 (0.75 0.05. A sizeable positive magnetoresistance is observed at low temperature which demonstrates that multiple MR mechanisms are possible in LnMnAsO oxypnictides.",1501.02996v1 2015-03-02,Functional Materials for Information and Energy Technology: Insights by Photoelectron Spectroscopy,"The evolution of both information and energy technology is intimately connected to complex condensed matter systems, the properties of which are determined by electronic and chemical interactions and processes on a broad range of length and time scales. Dedicated photoelectron spectroscopy and spectromicroscopy experiments can provide important insights. We discuss some recent methodological developments with application to relevant questions in spintronics, and towards in-operando studies of resistive switching and electrochemical processes.",1503.00464v2 2015-03-29,Cooperative Multiscale Aging in a Ferromagnet/Antiferromagnet Bilayer,"We utilize anisotropic magnetoresistance to study temporal evolution of the magnetization state in epitaxial Ni$_{80}$Fe$_{20}$/Fe$_{50}$Mn$_{50}$ ferromagnet/antiferromagnet bilayers. The resistance exhibits power-law evolution over a wide range of temperatures and magnetic fields, indicating that aging is characterized by a wide range of activation time scales. We show that aging is a cooperative process, i.e. the magnetic system is not a superposition of weakly interacting subsystems characterized by simple Arrhenius activation. The observed effects are reminiscent of avalanches in granular materials, providing a conceptual link to a broad class of critical phenomena in other complex condensed matter systems.",1503.08380v1 2015-11-17,On melting of boron phosphide under pressure,"Melting of cubic boron phosphide, BP has been studied at pressures to 9 GPa using synchrotron X-ray diffraction and electrical resistivity measurements. It has been found that above 2.6 GPa BP melts congruently, and the melting curve exhibits negative slope -60(7) K/GPa, which is indicative of a higher density of the melt as compared to the solid phase.",1511.05995v1 2015-11-30,Electronic Origins of Large Thermoelectric Power Factor of LaOBiS2-xSex,"We examined the electrical transport properties of densified LaOBiS2-xSex, which constitutes a new family of thermoelectric materials. The power factor increased with increasing concentration of Se, i.e., Se substitution led to an enhanced electrical conductivity, without suppression of the Seebeck coefficient. Hall measurements indicated that the low electrical resistivity resulted from increases in the carrier mobility, and the decrease in carrier concentration led to large absolute values of the Seebeck coefficient of the system.",1511.09133v1 2016-04-04,Two-dimensional Dirac fermions in YbMnBi2 antiferromagnet,"We report two-dimensional quantum transport and Dirac fermions in YbMnBi2 single crystals. YbMnBi2 is a layered material with anisotropic conductivity and magnetic order below 290 K. Magnetotransport properties, nonzero Berry phase and small cyclotron mass indicate the presence of quasi two dimensional Dirac fermions. Quantum oscillations in Hall resistivity suggest the presence of both electron and hole parts of the Fermi surface whereas the Berry phase suggests spin-orbit coupling.",1604.01009v1 2016-08-17,Field effect in stacked van der Waals heterostructures: Stacking sequence matters,"Stacked van der Waals (vdW) heterostructures where semi-conducting two-dimensional (2D) materials are contacted by overlayed graphene electrodes enable atomically-thin, flexible electronics. We use first-principles quantum transport simulations of graphene-contacted MoS2 devices to show how the transistor effect critically depends on the stacking configuration relative to the gate electrode. We can trace this behavior to the stacking-dependent response of the contact region to the capacitive electric field induced by the gate. The contact resistance is a central parameter and our observation establish an important design rule for devices based on 2D atomic crystals.",1608.05023v1 2017-06-30,Structural and dielectric characterization of Sm2MgMnO6,"The polycrystalline Sm2MgMnO6 (SMMO) was synthesized at 1173K by means of sol-gel technique. Rietveld refine-ment of X-ray diffraction (XRD) pattern confirmed the formation of a single phase monoclinic structure with space group P21/n. The band gap achieved from UV-vis spectra shows the semiconducting nature of the material. To observe the effect of grains and grain-boundaries in the conduction process and dielectric relaxation measurements are carried out on SMMO sample at different frequencies between 313 K and 673 K. An electrical equivalent circuit consisting of the resistance and constant phase element is used to clarify the impedance data.",1706.10038v1 2017-10-08,Hall effect spintronics for gas detection,"We present the concept of magnetic gas detection by the Extraordinary Hall effect (EHE). The technique is compatible with the existing conductometric gas detection technologies and allows simultaneous measurement of two independent parameters: resistivity and magnetization affected by the target gas. Feasibility of the approach is demonstrated by detecting low concentration hydrogen using thin CoPd films as the sensor material. The Hall effect sensitivity of the optimized samples exceeds 240% per 104 ppm at hydrogen concentrations below 0.5% in the hydrogen/nitrogen atmosphere, which is more than two orders of magnitude higher than the sensitivity of the conductance detection.",1710.03700v1 2017-10-12,Martensitic relief observation by atomic force microscopy in yttria stabilized zirconia,"The tetragonal to monoclinic (t-m) phase transformation of zirconia has been the object of extensive investigations of the last twenty years, and is now recognised as being of martensitic nature. However, martensitic transformation has only been observed by transmission electron microscopy or indirect methods. Though the benefit on the fracture toughness and crack resistance was the main interest, the transformation is now considered for its consequences on the degradation of the material. The use of AFM reported here allowed the observation of the first stages of martensite relief growth and of new martensitic features.",1710.04442v1 2017-10-25,Ordered C vacancies in titanium carbides: a correlation between crystal structure and the effects on oxidation behavior at elevated temperature,"It has been widely accepted that the introduction of titanium carbides into titanium-based alloys can significantly enhance the oxidation resistance due to their superior physicochemical stability at elevated temperatures. The present study reported for the first time that the ordered C vacancies within titanium carbides could lead to an uncommon phenomenon particularly at the very initial stage of oxidation. The intrinsic micro-to-macro oxidation mechanisms were systematically clarified with the aids of transmission electron microscope and ab-initio molecular dynamics simulation.",1710.09311v1 2017-12-28,Theoretical calculation of transport properties of oxide material using narrow band model,"We report about the results of theoretical calculations of temperature dependence of resistivity ($\rho$) and Seebeck coefficient ($S$) for thermoelectric (TE) and superconductivity (SC) phases by arithmetic equations based on narrow band model with oxygen deficient structure, as the functions of band-filling degree ($F$), and band width ratio of electron and spin states ($W$\sigma/$W$D). The phase diagrams of TE and SC states, and boundary were imaged to the properties of $\rho$ and $S$ as a function of $F$ and $W$\sigma/$W$D.",1712.09840v1 2018-01-12,Tunable elastic Parity-Time symmetric structure based on the shunted piezoelectric materials,"We theoretically and numerically report on tunable elastic Parity-Time (PT) symmetric structure based on shunted piezoelectric units. We show that the elastic loss and gain can be archived in piezoelectric materials when they are shunted by external circuits containing positive and negative resistances. We present and discuss, as an example, the strongly dependent relationship between the exceptional points of a three-layered system and the impedance of their external shunted circuit. The achieved results evidence the PT symmetric structures based on this proposed concept can actively be tuned without any change of their geometric configurations.",1801.04114v1 2018-02-12,Crack initiation in viscoelastic materials,"In viscoelastic materials, individually short-lived bonds collectively result in a mechanical resistance which is long-lived but finite, as ultimately cracks appear. Here we provide a microscopic mechanism by which cracks emerge from the nonlinear local bond dynamics. This mechanism is different from crack initiation in solids, which is governed by a competition between elastic and adhesion energy. We provide and numerically verify analytical equations for the dependence of the critical crack length on the bond kinetics and applied stress.",1802.04017v1 2017-01-27,Delicate competing electronic states in ultrathin manganite films,"The coupling between the electrical transport properties of La2/3Sr1/3MnO3 (LSMO) thin films and structural phase transitions of SrTiO3 (STO) substrates at Ts = 105 K has been investigated. We found that the electrical resistivity of LSMO films exhibit a cusp at Ts, which is greatly amplified by tuning films to the verge of metallic and insulating phases, i.e., to the boundary of two delicate competing electronic states. Our results demonstrate that small amounts of strain can tip the subtle balance of competing interactions and tune the electronic properties in correlated electron materials.",1701.07933v1 2019-07-03,Precision measurements of the AC field dependence of the superconducting transition in strontium titanate,"Strontium titanate has resurfaced as a material prompting vigorous debate about the origin of its superconductivity in the extremely low carrier concentration regime. Here, we used simultaneous AC susceptibility and transport methods to explore the superconducting phase transition region in this material. We determined that strontium titanate is extremely sensitive to even small AC fields, which also influence the resistive transition; we suggest that extreme vortex sizes and mobilities contribute to this large effect. Our findings will be of importance for accurately determining transition temperature, informing the debate about the pairing mechanism in strontium titanate, for which even millikelvin errors may be critical.",1907.01733v1 2020-04-14,Compaction Self-Assembly of Ultralow-Binder-Content Thermoplastic Composites Based on Lunar Soil Simulant,"In a recent study, we developed ultralow-binder-content (UBC) structural materials based on lunar soil simulant and thermoset binders. In the current research, we investigated thermoplastic binders. Compared to thermosets, advanced thermoplastics could be more UV resistant, more durable, more robust, and recyclable. Our main technology is the compaction self-assembly (CSA). By using only ~4 wt% polyetherketoneketone (PEKK) binder, the thermoplastic-binder UBC composite was stronger than typical steel-reinforced concrete. The CSA operation was separate from the curing process. This study may provide an important in-situ resource utilization method for large-scale construction on Moon.",2004.06273v1 2017-05-01,On melting of boron subnitride B13N2 under pressure,"Melting of rhombohedral boron subnitride B13N2 has been studied in situ at pressures to 8 GPa using synchrotron X-ray diffraction and electrical resistivity measurements. It has been found that above 2.6 GPa B13N2 melts incongruently, and the melting curve exhibits positive slope of 31(3) K/GPa that points to a lower density of the melt as compared to the solid phase.",1705.03753v1 2019-03-25,Optical Hoovering on Plasmonic Rinks,"Excitation of surface waves on conducting materials provides a near resistance-free interface capable of a material glissade either by plasmon forces or optical beam tractors. Analogous to an ice hockey rink, as proof of principle plasmon assisted optical traction, or hoovering, of water drops on a gold surface is demonstrated. Variability in thresholds and movement is observed and can be explained by the presence of significant roughness, measured by SEM. The demonstration opens a path to directly integrate various optical and plasmonic glissade technologies. Ways of improving transport and potential applications spanning configurable microfluidics, antennas, diagnostics,sensing and active devices are discussed.",1903.10106v1 2021-04-23,Microwave response in a topological superconducting quantum interference device,"Photon detection at microwave frequency is of great interest due to its application in quantum computation information science and technology. Herein are results from studying microwave response in a topological superconducting quantum interference device (SQUID) realized in Dirac semimetal Cd3As2. The temperature dependence and microwave power dependence of the SQUID junction resistance are studied, from which we obtain an effective temperature at each microwave power level. It is observed the effective temperature increases with the microwave power. This observation of microwave response may pave the way for single photon detection at the microwave frequency in topological quantum materials.",2104.11841v1 2021-04-29,Thickness Dependence of Magneto-transport Properties in Tungsten Ditelluride,"We investigate the electronic structure of tungsten ditelluride (WTe$_2$) flakes with different thicknesses in magneto-transport studies. The temperature-dependent resistance and magnetoresistance (MR) measurements both confirm the breaking of carrier balance induced by thickness reduction, which suppresses the `turn-on' behavior and large positive MR. The Shubnikov-de-Haas oscillation studies further confirm the thickness-dependent change of electronic structure of WTe$_2$ and reveal a possible temperature-sensitive electronic structure change. Finally, we report the thickness-dependent anisotropy of Fermi surface, which reveals that multi-layer WTe$_2$ is an electronic 3D material and the anisotropy decreases as thickness decreases.",2104.14464v1 2022-03-04,Impedance spectroscopy: Impedance spectroscopy of nanomaterials,"Solid state impedance spectroscopy enables the various contributions to the resistive and capacitive properties of electronically inhomogeneous condensed matter to be deconvoluted and characterized separately. The different contributions arise from electronically distinct areas in the sample, which can in an ideal case be represented each by one standard RC element. In the following, the basic principles of impedance spectroscopy, different types of experimental setups and several examples of experimental impedance data sets from nanostructured materials are reviewed and discussed. The data analysis and equivalent circuit modelling processes which are relevant for the application of this technique to nanomaterials are emphasized. The different dimensions and structure of nanomaterials as compared to macroscopic bulk samples leads to quite different and sometimes more complex data that require detailed analysis and advanced equivalent circuit models.",2203.02387v1 1998-12-08,Anomalous Low Temperature States in CeNi2Ge2,"Ambient pressure studies on high purity single crystals of the stoichiometric 4f-electron metal CeNi2Ge2 reveal anomalous low temperature forms of the resistivity which challenge our understanding of the metallic state. Comparisons are made with the isostructural and isoelectronic compound CePd2Si2 near the border of magnetism at high pressure, and possible reasons for this novel non-Fermi liquid form of the resistivity are discussed. Phase diagrams of further anomalies are presented, which involve a loss of resistance at low temperature in some samples of CeNi2Ge2 and unexpected high pressure phases.",9812133v1 2003-03-20,Electrical resistivity and magnetization measurements on the heavy fermion superconductor PrOs4Sb12,"The filled skutterudite compound PrOs4Sb12, the first example of a Pr-based heavy fermion superconductor, displays superconductivity with $T_c\sim 1.85$ K and has an effective mass $m^* \sim$ {50 $m_e$}, where $m_e$ is the free electron mass. For magnetic fields above 4.5 T, sharp features in the normal state electrical resistivity, magnetization, specific heat, and thermal expansion data suggest the occurrence of a phase transition at high fields. This high field ordered phase in the normal state may originate from a combination of crystalline electric field enhanced Zeeman splitting and quadrupolar ordering. We present an investigation of the electrical resistivity and magnetization of PrOs4Sb12 as a function of temperature between {350 mK} and {3.5 K} and magnetic field up to {18 T}. The data reveal a detailed phase boundary of the high field ordered phase as well as the lower critical field $H_{c1}$ and the onset field of the peak effect in the superconducting state of PrOs4Sb12.",0303405v1 2004-04-12,Universality of the Mott-Ioffe-Regel limit in metals,"The absence of resistivity saturation in many strongly correlated metals, including the high-temperature superconductors, is critically examined from the viewpoint of optical conductivity measurements. Coherent quasiparticle conductivity, in the form of a Drude peak centred at zero frequency, is found to disappear as the mean free path (at $\omega$ = 0) becomes comparable to the interatomic spacing. This basic loss of coherence at the so-called Mott-Ioffe-Regel (MIR) limit suggests that the universality of the MIR criterion is preserved even in the presence of strong electron correlations. We argue that the shedding of spectral weight at low frequencies, induced by strong correlation effects, is the primary origin of the extended positive slope of the resistivity to high temperatures observed in all so-called ""bad metals"". Moreover, in common with those metals which exhibit resistivity saturation at high temperatures, the scattering rate itself, as extracted from optical spectra, saturates at a value consistent with the MIR limit. We consider possible implications that this ceiling in the scattering rate may have for our understanding of transport within a wide variety of bad metals and suggest a better method for analysing their optical response.",0404263v1 2005-02-21,High pressure effects on the superconductivity of beta-pyrochlore oxides AOs2O6,"High pressure effects on the superconducting transitions of beta-pyrochlore superconductors AOs2O6 (A = Cs, Rb, K) are studied by measuring resistivity under high pressures up to 10 GPa. The superconducting transition temperature Tc first increases with increasing pressure in all the compounds and then exhibits a broad maximum at 7.6 K (6 GPa), 8.2 K (2 GPa) and 10 K (0.6 GPa) for A = Cs, Rb and K, respectviely. Finally, the superconductivity is suppressed completely at a critical pressure near 7 GPa and 6 GPa for A = Rb and K and probably above 10 GPa for A = Cs. Characteristic changes in the coefficinet A of the T2 term in resistivity and residual resistivity are observed, both of which are synchronized with the corresponding change in Tc. It is suggested that electron correlations and certain quantum fluctuations play important roles in the occurrence or suppression of superconductivity in the beta-pyrochlore oxides.",0502490v1 2003-07-30,Position Sensing from Charge Dispersion in Micro-Pattern Gas Detectors with a Resistive Anode,"Micro-pattern gas detectors, such as the Gas Electron Multiplier (GEM) and the Micromegas need narrow high density anode readout elements to achieve good spatial resolution. A high-density anode readout would require an unmanageable number of electronics channels for certain potential micro-detector applications such as the Time Projection Chamber. We describe below a new technique to achieve good spatial resolution without increasing the electronics channel count in a modified micro-detector outfitted with a high surface resistivity anode readout structure. The concept and preliminary measurements of spatial resolution from charge dispersion in a modified GEM detector with a resistive anode are described below.",0307152v2 2008-09-30,High Pressure studies of the magnetic phase transition in MnSi: revisited,"New measurements of AC magnetic susceptibility and DC resistivity of a high quality single crystal MnSi were carried out at high pressure making use of helium as a pressure medium. The form of the AC magnetic susceptibility curves at the magnetic phase transition suddenly changes upon helium solidification. This implies strong sensitivity of magnetic properties of MnSi to non hydrostatic stresses and suggests that the early claims on the existence of a tricritical point at the phase transition line are probably a result of misinterpretation of the experimental data. At the same time resistivity behavior at the phase transition does not show such a significant influence of helium solidification. The sharp peak at the temperature derivative of resistivity, signifying the first order nature of the phase transition in MnSi successfully survived helium crystallization and continued the same way to the highest pressure.",0809.5117v1 2014-05-21,Waveguide-mode interference lithography technique for high contrast subwavelength structures in the visible region,"We explore possibilities of waveguide-mode interference lithography (WMIL) technique for high contrast subwavelength structures in the visible region. Selecting an appropriate waveguide-mode, we demonstrate high contrast resist mask patterns for the first time. TM1 mode in the waveguide is shown to be useful for providing a three-dimensional structure whose cross section is checkerboard pattern. Applying our WMIL technique, we demonstrate 1D, 2D and 3D subwavelength resist patterns that are widely used for the fabrication of metamteterials in the visible region. In addition to the resist patterns, we demonstrate a resonance at 1.9 eV for a split tube structure experimentally.",1405.5395v1 2015-10-28,Effect of ambient on the resistance fluctuations of graphene,"In this letter we present the results of systematic experimental investigations of the effect of different chemical environments on the low frequency resistance fluctuations of single layer graphene field effect transistors (SLG-FET). The shape of the power spectral density of noise was found to be determined by the energetics of the adsorption-desorption of molecules from the graphene surface making it the dominant source of noise in these devices. We also demonstrate a method of quantitatively determining the adsorption energies of chemicals on graphene surface based on noise measurements. We find that the magnitude of noise is extremely sensitive to the nature and amount of the chemical species present. We propose that a chemical sensor based on the measurement of low frequency resistance fluctuations of single layer graphene field effect transistor devices will have extremely high sensitivity, very high specificity, high fidelity and fast response times.",1510.08198v1 2016-07-09,In-beam evaluation of a medium-size Resistive-Plate WELL gaseous particle detector,"In-beam evaluation of a fully-equipped medium-size 30$\times$30 cm$^2$ Resistive Plate WELL (RPWELL) detector is presented. It consists here of a single element gas-avalanche multiplier with Semitron ESD225 resistive plate, 1 cm$^2$ readout pads and APV25/SRS electronics. Similarly to previous results with small detector prototypes, stable operation at high detection efficiency (>98%) and low average pad multiplicity (~1.2) were recorded with 150 GeV muon and high-rate pion beams, in Ne/(5%CH$_4$), Ar/(5%CH$_4$) and Ar/(7%CO$_2$). This is an important step towards the realization of robust detectors suitable for applications requiring large-area coverage; among them Digital Hadron Calorimetry.",1607.02587v2 2017-12-26,Microwave-induced zero-resistance states in a high-mobility two-subband electron system,"In this study we used selectively-doped GaAs/AlAs heterostructure to fabricate a high-mobility two-subband electronic system with substantially different concentration of electrons in subbands. We observe microwave photoresistance at high numbers of magneto-intersubband oscillations (MISO). The system under study demonstrates microwave-induced resistance oscillations (MIRO) and MISO interference. MIRO in the studied two-subband system appear in lower magnetic fields comparing to MISO. This is an indication of some unknown mechanism that exists in the two-subband system and is responsible for MISO amplitude damping in low magnetic fields, while it does not affect the MIRO amplitude. Zero resistance states (ZRS) appear in the system under study under microwave irradiation in the narrow range of magnetic fields near the MISO maximum.",1712.09244v1 2020-04-11,Characterisation of an RPC prototype with moderate resistivity plates using tetrafluoroethane ($C_2H_2F_4$),"Keeping in mind the requirements of high rate capable, cost effective, large area detectors to be used in future high energy physics experiments, commercially available bakelite plates having moderate bulk resistivity are used to build an RPC module. The chamber is tested with cosmic rays in the avalanche mode using 100\% Tetrafluoroethane ($C_2H_2F_4$). Standard NIM electronics are used for this study. The efficiency, noise rate and time resolution are measured. The detailed method of measurement and the first test results are presented.",2004.05469v2 2019-08-29,Onset of phase diffusion in high kinetic inductance granular aluminum micro-SQUIDs,"Superconducting granular aluminum is attracting increasing interest due to its high kinetic inductance and low dissipation, favoring its use in kinetic inductance particle detectors, superconducting resonators or quantum bits. We perform switching current measurements on DC-SQUIDs, obtained by introducing two identical geometric constrictions in granular aluminum rings of various normal-state resistivities in the range from $\rho_\mathrm{n} = 250\,\mu\Omega\mathrm{cm}$ to $5550\,\mu\Omega\mathrm{cm}$. The relative high kinetic inductance of the SQUID loop, in the range of tens of nH, leads to a suppression of the modulation in the measured switching current versus magnetic flux, accompanied by a distortion towards a triangular shape. We observe a change in the temperature dependence of the switching current histograms with increasing normal-state film resistivity. This behavior suggests the onset of a diffusive motion of the superconducting phase across the constrictions in the two-dimensional washboard potential of the SQUIDs, which could be caused by a change of the local electromagnetic environment of films with increasing normal-state resistivities.",1908.11067v1 2019-12-18,"Multiplex stimulated Raman scattering imaging cytometry reveals cancer metabolic signatures in a spatially, temporally, and spectrally resolved manner","In situ measurement of cellular metabolites is still a challenge in biology. Conventional methods, such as mass spectrometry or fluorescence microscopy, would either destruct the sample or introduce strong perturbations to the functions of target molecules. Here, we present multiplex stimulated Raman scattering (SRS) imaging cytometry as a label-free single-cell analysis platform with chemical specifity, and high-throughput capabilities. Cellular compartments such as lipid droplets, endoplasmic reticulum, and nuclei are seperated from the cytoplasm. Based on these chemical segmentations, 260 features from both morphology and molecular composition were generated and analyzed for each cell. Using SRS imaging cytometry, we studied the metabolic responses of human pancreatic cancer cells under stress by starvation and chemotherapy drug treatments. We unveiled lipid-facilitated protrusion as a metabolic marker for stress-resistant cancer cells through statistical analysis of thousands of cells. Our findings also demonstrate the potential of targeting lipid metabolism for selective treatment of starvation-resistant and chemotherapy-resistant cancers. These results highlight our SRS imaging cytometry as a powerful label-free tool for biological discoveries with a high-throughput, high-content capacity.",1912.08340v1 2020-05-31,Towards a two-dimensional readout of the improved CMS Resistive Plate Chamber with a new front-end electronics,"As part of the Compact Muon Solenoid experiment Phase-II upgrade program, new Resistive Plate Chambers will be installed in the forward region. High background conditions are expected in this region during the high-luminosity phase of the Large Hadron Collider, therefore an improved RPC design has been proposed with a new front-end electronics to sustain a higher rate capability and better time resolution. A new technology is used in the front-end electronics resulting in very low achievable thresholds of the order of several fC. Crucial in the design of the improved RPC is the capability of a two-dimensional readout in order to improve the spatial resolution, mainly motivated by trigger requirements. In this work, the first performance results towards this two-dimensional readout are presented, based on data taken on a real-size prototype chamber with two embedded orthogonal readout strips. Furthermore, dedicated studies of the muon cluster size as a function of the graphite resistivity are discussed.",2006.00576v1 2020-06-24,Microwave response of interacting oxide two-dimensional electron systems,"We present an experimental study on microwave illuminated high mobility MgZnO/ZnO based two-dimensional electron systems with different electron densities and, hence, varying Coulomb interaction strength. The photoresponse of the low-temperature dc resistance in perpendicular magnetic field is examined in low and high density samples over a broad range of illumination frequencies. In low density samples a response due to cyclotron resonance (CR) absorption dominates, while high density samples exhibit pronounced microwave-induced resistance oscillations (MIRO). Microwave transmission experiments serve as a complementary means of detecting the CR over the entire range of electron densities and as a reference for the band mass unrenormalized by interactions. Both CR and MIRO-associated features in the resistance permit extraction of the effective mass of electrons but yield two distinct values. The conventional cyclotron mass representing center-of-mass dynamics exhibits no change with density and coincides with the band electron mass of bulk ZnO, while MIRO mass reveals a systematic increase with lowering electron density consistent with renormalization expected in interacting Fermi liquids.",2006.13627v1 2020-10-15,Extreme High-Field Superconductivity in Thin Re Films,"We report the high-field superconducting properties of thin, disordered Re films via magneto-transport and tunneling density of states measurements. Films with thicknesses in the range of 9 nm to 3 nm had normal state sheet resistances of $\sim$0.2 k$\Omega$ to $\sim$1 k$\Omega$ and corresponding transition temperatures in the range of 6 K to 3 K. Tunneling spectra were consistent with those of a moderate coupling BCS superconductor. Notwithstanding these unremarkable superconducting properties, the films exhibited an extraordinarily high upper critical field. We estimate their zero-temperature $H_{c2}$ to be more than twice the Pauli limit. Indeed, in 6 nm samples the estimated reduced critical field $H_{c2}/T_c\sim$ 5.6 T/K is among the highest reported for any elemental superconductor. Although the sheet resistances of the films were well below the quantum resistance $R_Q=h/4e^2$, their $H_{c2}$'s approached the theoretical upper limit of a strongly disordered superconductor for which $k_F\ell\sim1$.",2010.07674v2 2021-09-29,High-performance Ba1-xKxFe2As2 superconducting joints for persistent current operation,"Superconducting joints are one of the key technologies to make Ba1-xKxFe2As2 (Ba-122) superconducting wires or tapes for high-field applications. Herein, superconducting joints were fabricated by a simple cold-pressing method, and the joint resistance of the iron-based superconducting joint was estimated for the first time. The superconducting properties, microstructures, and elements distribution in the joint regions were investigated. At 4.2 K and 10 T, a transport critical current Ic of 105 A for the joint was obtained, and the critical current ratio (CCR= Ic-joint/Ic-tape) of the joint was 94.6%. On the other hand, the joint show very low joint resistance of 2.7x10^-13 ohm in self-field at 4.2 K. Among iron-based superconductors (IBS), this work is the first to successfully realize a superconducting joint with such high CCR and low joint resistance. This work shows great potential to apply Ba-122 in a range of practical applications, where superconducting joints are essential.",2109.14300v1 2022-09-01,Directed flow in relativistic resistive magneto-hydrodynamic expansion for symmetric and asymmetric collision systems,"We construct a dynamical model for high-energy heavy-ion collision based on the relativistic resistive magneto-hydrodynamic framework. Using our newly developed (3+1)-dimensional relativistic resistive magneto-hydrodynamics code, we investigate magneto-hydrodynamic expansion in symmetric and asymmetric collision systems as a first application to high-energy heavy-ion collisions. As a realistic initial condition for electromagnetic fields, we consider the solutions of the Maxwell equations with the source term of point charged particles moving in the direction of the beam axis, including finite constant electrical conductivity of the medium. We evaluate the directed flow in the symmetric and asymmetric collisions at RHIC energy. We find a significant effect of finite electrical conductivity on the directed flow in the asymmetric collision system. We confirm that a certain amount of energy transfer by dissipation associated with Ohmic conduction occurs in the asymmetric collision system because of asymmetry of the electric field produced by two different colliding nuclei. Because this energy transfer makes the pressure gradient of the medium flatter, the growth of directed flow decreases.",2209.00323v1 2023-02-21,A novel fast response and radiation-resistant scintillator detector for beam loss monitor,"At high luminosity areas, beam loss monitor with fast response and high radiation resistance is crucial for accelerator operation. In this article, we report the design and test results of a fast response and radiation-resistant scintillator detector as the beam loss monitor for high luminosity colliders, especially at low energy regions such as RFQ. The detector consists of a 2 cm*2 cm 0.5 cm LYSO crystal readout by a 6 mm*6 mm Silicon photomultiplier. Test results from various radioactive sources show that the detector has good sensitivity to photons from tens of keV to several MeV with good linearity and energy resolution (23% for 60 keV {\gamma}-ray). For the field test, two such detectors are installed outside of the vacuum chamber shell of an 800 MeV electron storage ring. The details of the test and results are introduced.",2302.14662v1 2023-11-28,Transport properties of a half-filled Chern band at the electron and composite fermion phases,"We consider a half-filled Chern band and its transport properties in two phases that it may form, the electronic Fermi liquid and the composite-fermion Fermi liquid. For weak disorder, we show that the Hall resistivity for the former phase is very small, while for the latter it is close to $2h/e^2$, independent of the distribution of the Berry curvature in the band. At rising temperature and high frequency, we expect the Hall resistivity of the electronic phase to rise, and that of the composite-fermion phase to deviate from $2h/e^2$. At high frequency, sign changes are expected as well. Considering high-frequency transport, we show that the composite fermion phase carries a gapped plasmon mode which does not originate from long ranged Coulomb interaction, and we show how this mode, together with the reflection of electro-magnetic waves off the Chern band, allow for a measurement of the composite-fermion Drude weight and Berry curvature. Finally, we consider a scenario of a mixed-phase transition between the two phases, for example as a function of displacement-field, and show that such transition involves an enhancement of the longitudinal resistivity, as observed experimentally.",2311.16761v1 2024-05-17,Possible spin-polarized Cooper pairing in high temperature FeSe superconductor,"Superconductivity and long-range ferromagnetism hardly coexist in a uniform manner. The counter-example has been observed, in uranium-based superconductors for instance, with a coexisting temperature limited to about 1 K. Here, we report the coexistence of high temperature superconductivity and itinerant ferromagnetism in lithium intercalated FeSe flakes. In superconducting samples with transition temperature around 40 K, we observe the anomalous Hall effect with a hysteresis loop in transverse resistivity and a butterfly-like pattern of magneto-resistance. Intriguingly, such ferromagnetism persists down to a temperature at which the zero-field resistance fully vanishes. Furthermore, the superconductivity is enhanced under an in-plane magnetic field, suggestive of the participation of spin-polarized Cooper pairs. The surprising finding underscores a uniform coexistence of the two antagonistic phenomena on a record-high energy scale.",2405.10482v1 2006-05-24,Tuning of magnetic and electronic states by control of oxygen content in lanthanum strontium cobaltites,"We report on the magnetic, resistive, and structural studies of perovskite La$_{1/3}$Sr$_{2/3}$CoO$_{3-\delta}$. By using the relation of synthesis temperature and oxygen partial pressure to oxygen stoichiometry obtained from thermogravimetric analysis, we have synthesized a series of samples with precisely controlled $\delta=0.00-0.49$. These samples show three structural phases at $\delta=0.00-0.15$, $\approx0.25$, $\approx0.5$, and two-phase behavior for other oxygen contents. The stoichiometric material with $\delta=0.00$ is a cubic ferromagnetic metal with the Curie temperature $T_{\rm C}=274$ K. The increase of $\delta$ to 0.15 is followed by a linear decrease of $T_{\rm C}$ to $\approx$ 160 K and a metal-insulator transition near the boundary of the cubic structure range. Further increase of $\delta$ results in formation of a tetragonal $2a_p\times 2a_p \times 4a_p$ phase for $\delta\approx 0.25$ and a brownmillerite phase for $\delta\approx0.5$. At low temperatures, these are weak ferromagnetic insulators (canted antiferromagnets) with magnetic transitions at $T_{\rm m}\approx230$ and 120 K, respectively. At higher temperatures, the $2a_p\times 2a_p \times 4a_p$ phase is $G$-type antiferromagnetic between 230 K and $\approx$360 K. Low temperature magnetic properties of this system for $\delta<1/3$ can be described in terms of a mixture of Co$^{3+}$ ions in the low-spin state and Co$^{4+}$ ions in the intermediate-spin state and a possible spin transition of Co$^{3+}$ to the intermediate-spin state above $T_{\rm C}$. For $\delta>1/3$, there appears to be a combination of Co$^{2+}$ and Co$^{3+}$ ions, both in the high-spin state with dominating antiferromagnetic interactions.",0605611v1 2008-06-23,"Phase transitions in LaFeAsO: structural, magnetic, elastic, and transport properties, heat capacity and Mossbauer spectra","We present results from a detailed experimental investigation of LaFeAsO, the parent material in the series of ""FeAs"" based oxypnictide superconductors. Upon cooling this material undergoes a tetragonal-orthorhombic crystallographic phase transition at ~160 K followed closely by an antiferromagnetic ordering near 145 K. Analysis of these phase transitions using temperature dependent powder X-ray and neutron diffraction measurements is presented. A magnetic moment of ~0.35 Bohr magnetons per iron is derived from Mossbauer spectra in the low temperature phase. Evidence of the structural transition is observed at temperatures well above the structural transition (up to near 200 K) in the diffraction data as well as the polycrystalline elastic moduli probed by resonant ultrasound spectroscopy measurements. The effects of the two phase transitions on the transport properties (resistivity, thermal conductivity, Seebeck coefficient, Hall coefficient), heat capacity, and magnetization of LaFeAsO are also reported, including a dramatic increase in the magnitude of the Hall coefficient below 160 K. The results suggest that the structural distortion leads to a localization of carriers on Fe, producing small local magnetic moments which subsequently order antiferromagnetically upon further cooling. Evidence of strong electron-phonon interactions in the high-temperature tetragonal phase is also observed.",0806.3878v2 2011-03-07,Reversibly tuning the insulating and superconducting state in KxFe2-ySe2 crystals by post-annealing,"Since the discovery of superconductivity at 26 K in oxy-pnictide LaFeAsO1-xFx, enormous interests have been stimulated in the field of condensed matter physics and material sciences. Among the many kind of structures in the iron pnictide superconductors, FeSe with the PbO structure has received special attention since there is not poisonous pnictogen element in chemical composition and its structure is the simplest one. However, the superconducting transition temperature (Tc) in iron chalcogenide compounds is not enhanced as high as other iron pnictide superconductors under ambient pressure until the superconductivity at above 30 K in potassium intercalated iron selenide KxFe2-ySe2 was discovered. The insulating and the superconducting state are both observed in KxFe2-ySe2 with different stoichiometries and some groups have tuned the system from insulating to superconducting state by varying the ratio of starting materials[10, 11]. The recent data from neutron scattering suggest that the superconductivity may be built upon an ordered state of Fe vacancies as well as the antiferromagnetic state with a very strong ordered magnetic moment 3.4 B. Here we show that the superconductivity can actually be tuned on a single sample directly from an insulating state by post-annealing and fast quenching. Upon waiting for some days at room temperatures, the superconductivity will disappear and the resistivity exhibits an insulating behavior again. The spatial distribution of the compositions of the as-grown sample and the post-annealed-quenched one was analyzed by the Energy Dispersive X-ray Spectrum (EDXS) and found to be very close to each other. Therefore it is tempting to conclude that the superconductivity is achieved when the Fe-vacancies are in a random (disordered) state. Once they arrange in an ordered state by relaxation or slow cooling, the system turns out to be an insulator.",1103.1347v1 2014-09-16,Hydrogen Diffusion and Stabilization in Single-crystal VO2 Micro/nanobeams by Direct Atomic Hydrogenation,"We report measurements of the diffusion of atomic hydrogen in single crystalline VO2 micro/nanobeams by direct exposure to atomic hydrogen, without catalyst. The atomic hydrogen is generated by a hot filament, and the doping process takes place at moderate temperature (373 K). Undoped VO2 has a metal-to-insulator phase transition at ~340 K between a high-temperature, rutile, metallic phase and a low-temperature, monoclinic, insulating phase with a resistance exhibiting a semiconductor-like temperature dependence. Atomic hydrogenation results in stabilization of the metallic phase of VO2 micro/nanobeams down to 2 K, the lowest point we could reach in our measurement setup. Based on observing the movement of the hydrogen diffusion front in single crystalline VO2 beams, we estimate the diffusion constant for hydrogen along the c-axis of the rutile phase to be 6.7 x 10^{-10} cm^2/s at approximately 373 K, exceeding the value in isostructural TiO2 by ~ 38x. Moreover, we find that the diffusion constant along the c-axis of the rutile phase exceeds that along the equivalent a-axis of the monoclinic phase by at least three orders of magnitude. This remarkable change in kinetics must originate from the distortion of the ""channels"" when the unit cell doubles along this direction upon cooling into the monoclinic structure. Ab initio calculation results are in good agreement with the experimental trends in the relative kinetics of the two phases. This raises the possibility of a switchable membrane for hydrogen transport.",1409.4661v1 2012-01-04,Synthesis and physical properties of the new potassium iron selenide superconductor K0.80Fe1.76Se2,"In this article we review our studies of the K0.80Fe1.76Se2 superconductor, with an attempt to elucidate the crystal growth details and basic physical properties over a wide range of temperatures and applied magnetic field, including anisotropic magnetic and electrical transport properties, thermodynamic, London penetration depth, magneto-optical imaging and Mossbauer measurements. We find that: (i) Single crystals of similar stoichiometry can be grown both by furnace-cooled and decanted methods; (ii) Single crystalline K0.80Fe1.76Se2 shows moderate anisotropy in both magnetic susceptibility and electrical resistivity and a small modulation of stoichiometry of the crystal, which gives rise to broadened transitions; (iii) The upper critical field, Hc2(T) is ~ 55 T at 2 K for H||c, manifesting a temperature dependent anisotropy that peaks near 3.6 at 27 K and drops to 2.5 by 18 K; (iv) Mossbauer measurements reveal that the iron sublattice in K0.80Fe1.76Se2 clearly exhibits magnetic order, probably of the first order, from well below Tc to its Neel temperature of Tn = 532 +/- 2 K. It is very important to note that, although, at first glance there is an apparent dilemma posed by these data: high Tc superconductivity in a near insulating, large ordered moment material, analysis indicates that the sample may well consist of two phases with the minority superconducting phase (that does not exhibit magnetic order) being finely distributed, but connected with in an antiferromagnetic, poorly conducting, matrix, essentially making a superconducting aerogel.",1201.0953v2 2019-04-24,Role of Oxygen Adsorption in Nanocrystalline ZnO Interfacial Layers for Polymer-Fullerene Bulk Heterojunction Solar Cells,"Colloidal zinc oxide (ZnO) nanoparticles are frequently used in the field of organic photovoltaics for the realization of solution-producible, electron-selective interfacial layers. Despite of the widespread use, there is a lack of detailed investigations regarding the impact of structural properties of the particles on the device performance. In this work, ZnO nanoparticles with varying surface-area-to-volume ratio were synthesized and implemented into polymer-fullerene bulk heterojunction solar cells with a gas-permeable top electrode. By comparing the electrical characteristics before and after encapsulation, it was found that the internal surface area of the ZnO layer plays a crucial role under conditions where oxygen can penetrate the solar cells. The adsorption of oxygen species at the nanoparticle surface causes band bending and electron depletion next to the surface. Both effects result in the formation of a barrier for electron injection and extraction at the ZnO/bulk heterojunction interface and were more pronounced in case of small ZnO nanocrystals (high surface-area-to-volume ratio). Different transport-related phenomena in the presence of oxygen are discussed in detail, i.e., Ohmic losses, expressed in terms of series resistance, as well as the occurrence of space-charge-limited currents, related to charge accumulation in the polymer-fullerene blend. Since absorption of UV light can cause desorption of adsorbed oxygen species, the electrical properties depend also on the illumination conditions. With the help of systematic investigations of the current versus voltage characteristics of solar cells under different air exposure and illumination conditions as well as studies of the photoconductivity of pure ZnO nanoparticle layers, we gain detailed insight into the role of the ZnO nanoparticle surface for the functionality of the organic solar cells.",1904.10916v1 2020-10-12,Landau Quantization and Highly Mobile Fermions in an Insulator,"In strongly correlated materials, quasiparticle excitations can carry fractional quantum numbers. An intriguing possibility is the formation of fractionalized, charge-neutral fermions, e.g., spinons and fermionic excitons, that result in neutral Fermi surfaces and Landau quantization in an insulator. While previous experiments in quantum spin liquids, topological Kondo insulators, and quantum Hall systems have hinted at charge-neutral Fermi surfaces, evidence for their existence remains far from conclusive. Here we report experimental observation of Landau quantization in a two dimensional (2D) insulator, i.e., monolayer tungsten ditelluride (WTe$_{2}$), a large gap topological insulator. Using a detection scheme that avoids edge contributions, we uncover strikingly large quantum oscillations in the monolayer insulator's magnetoresistance, with an onset field as small as ~ 0.5 tesla. Despite the huge resistance, the oscillation profile, which exhibits many periods, mimics the Shubnikov-de Haas oscillations in metals. Remarkably, at ultralow temperatures the observed oscillations evolve into discrete peaks near 1.6 tesla, above which the Landau quantized regime is fully developed. Such a low onset field of quantization is comparable to high-mobility conventional two-dimensional electron gases. Our experiments call for further investigation of the highly unusual ground state of the WTe$_{2}$ monolayer. This includes the influence of device components and the possible existence of mobile fermions and charge-neutral Fermi surfaces inside its insulating gap.",2010.05383v2 2021-07-29,Shearing Mechanisms of Co-Precipitates in IN718,"The Ni-base superalloy 718 is the most widely used material for turbomachinery in the aerospace industry and land-based turbines. Although the relationship between processing and the resulting properties is well known, an understanding of the specific deformation mechanisms activated across its application temperature range is required to create more mechanistically accurate property models. Direct atomic-scale imaging observations with high angle annular dark-field scanning transmission electron microscopy, complemented by phase-field modeling informed by generalized stacking fault surface calculations using density functional theory, were employed to understand the shear process of ${\gamma}''$ and ${\gamma}'/{\gamma}''$ co-precipitates after 1 \% macroscopic strain at lower temperature (ambient and $427 {\deg}C$). Experimentally, intrinsic stacking faults were observed in the ${\gamma}''$, whereas the ${\gamma}'$ was found to exhibit anti-phase boundaries or superlattice intrinsic stacking faults. Additionally, the atomically flat ${\gamma}'/{\gamma}''$ interfaces in the co-precipitates were found to exhibit offsets after shearing, which can be used as tracers for the deformation events. Phase-field modeling shows that the developing fault-structure is dependent on the direction of the Burgers vector of the $a/2 \langle110\rangle$ matrix dislocation (or dislocation group) due to the lower crystal symmetry of the ${\gamma''}$ phase. The interplay between ${\gamma}'$ and ${\gamma}''$ phases results in unique deformation pathways of the co-precipitate and increases the shear resistance. Consistent with the experimental observations, the simulation results indicate that complex shearing mechanisms are active in the low-temperature deformation regime and that multiple $a/2 \langle110\rangle$ dislocations of non-parallel Burgers vectors may be active on the same slip plane.",2107.13840v1 2021-08-24,In Situ Photothermal Response of Single Gold Nanoparticles Through Hyperspectral Imaging AntiStokes Thermometry,"Several fields of applications require a reliable characterization of the photothermal response and heat dissipation of nanoscopic systems, which remains a challenging task both for modeling and experimental measurements. Here, we present a new implementation of anti-Stokes thermometry that enables the in situ photothermal characterization of individual nanoparticles (NPs) from a single hyperspectral photoluminescence confocal image. The method is label-free, applicable to any NP with detectable anti-Stokes emission, and does not require any prior information about the NP itself or the surrounding media. With it, we first studied the photothermal response of spherical gold NPs of different sizes on glass substrates, immersed in water, and found that heat dissipation is mainly dominated by the water for NPs larger than 50 nm. Then, the role of the substrate was studied by comparing the photothermal response of 80 nm gold NPs on glass with sapphire and graphene, two materials with high thermal conductivity. For a given irradiance level, the NPs reach temperatures 18% lower on sapphire and 24% higher on graphene than on bare glass. The fact that the presence of a highly conductive material such as graphene leads to a poorer thermal dissipation demonstrates that interfacial thermal resistances play a very significant role in nanoscopic systems, and emphasize the need for in situ experimental thermometry techniques. The developed method will allow addressing several open questions about the role of temperature in plasmon-assisted applications, especially ones where NPs of arbitrary shapes are present in complex matrixes and environments.",2108.10954v1 2022-01-10,Superior enhancement in thermal conductivity of epoxy/graphene nanocomposites through use of dimethylformamide (DMF) relative to acetone as solvent,"In this work, we demonstrate that use of dimethylformamide (DMF) as a solvent leads to better dispersion of graphene nanoplatelets in epoxy matrix compared to acetone solvent, in turn leading to higher thermal conductivity epoxy-graphene nanocomposites. While role of solvents in enabling superior mechanical properties has been addressed before, outlined study is the first to address the effect of solvents on thermal conductivity enhancement and provides novel pathways for achieving high thermal conductivity polymer composite materials. Uniform dispersion of graphene nanoparticles into epoxy can improve thermal contact with polymer leading to superior interface thermal conductance between polymer matrix and graphene. Organic solvents are typically employed to achieve efficient dispersion of graphene into the epoxy matrix. In this study, we compare the effect of two organic solvents, dimethylformamide (DMF) and acetone, in terms of their efficiency in dispersing graphene into the epoxy matrix and their effect on enhancing thermal conductivity of the composite. We find that polymer-graphene composites made with DMF solvent show 44% higher thermal conductivity compared to those made using acetone at 7 weight% filler composition. Laser scanning confocal microscopy (LSCM) imaging reveals that graphene-epoxy composites, prepared using DMF as solvent, exhibit more uniform dispersion of graphene-nanoplatelets compared to the case of acetone with acetone-based samples exhibiting up to 211% larger graphene agglomerations. Comparison with effective medium theory reveals an almost 35% lower interface thermal resistance between graphene and epoxy for DMF relative to acetone prepared composite. These results provide fundamentally new avenues to achieve higher thermal conductivity graphene-epoxy composites, of key importance for a wide range of thermal management technologies.",2201.03527v2 2022-04-15,Universal Non-Polar Switching in Carbon-doped Transition Metal Oxides (TMOs) and Post TMOs,"Transition metal oxides (TMOs) and post-TMOs (PTMOs), when doped with Carbon, show non-volatile current-voltage (I-V) characteristics, which are both universal and repeatable. We have shown spectroscopic evidence of the introduction of carbon-based impurity states inside the existing larger bandgap effectively creating a smaller bandgap which we suggest could enable Mott-like correlation effect. Our findings indicate new insights for yet to be understood unipolar and nonpolar resistive switching in the TMOs and PTMOs. We have shown that device switching is not thermal-energy dependent and have developed an electronic-dominated switching model that allows for the extreme temperature operation (from 1.5 K to 423 K) and state retention up to 673 K for a 1-hour bake. Importantly, we have optimized the technology in an industrial process and demonstrated integrated 1-transistor/1-resistor (1T1R) arrays up to 1 kbit with 47 nm devices on 300 mm wafers for advanced node CMOS-compatible correlated electron RAM (CeRAM). These devices are shown to operate with 2 ns write pulses and retain the memory states up to 200 C for 24 hours. The collection of attributes shown, including scalability to state-of-the-art dimensions, non-volatile operation to extreme low and high temperatures, fast write, and reduced stochasticity as compared to filamentary memories such as ReRAMs show the potential for a highly capable two-terminal back-end-of-line non-volatile memory.",2204.07656v1 2022-07-18,Room temperature spin-orbit torque efficiency in sputtered low-temperature superconductor delta-TaN,"In the course of searching for promising topological materials for applications in future topological electronics, we evaluated spin-orbit torques (SOTs) in high-quality sputtered ${\delta}-$TaN/Co20Fe60B20 devices through spin-torque ferromagnetic resonance ST-FMR and spin pumping measurements. From the ST-FMR characterization we observed a significant linewidth modulation in the magnetic Co20Fe60B20 layer attributed to the charge-to-spin conversion generated from the ${\delta}-$TaN layer. Remarkably, the spin-torque efficiency determined from ST-FMR and spin pumping measurements is as large as ${\Theta} =$ 0.034 and 0.031, respectively. These values are over two times larger than for ${\alpha}-$Ta, but almost five times lower than for ${\beta}-$Ta, which can be attributed to the low room temperature electrical resistivity $\sim 74{\mu}{\Omega}$ cm in ${\delta}-$TaN. A large spin diffusion length of at least $\sim8$ nm is estimated, which is comparable to the spin diffusion length in pure Ta. Comprehensive experimental analysis, together with density functional theory calculations, indicates that the origin of the pronounced SOT effect in ${\delta}-$TaN can be mostly related to a significant contribution from the Berry curvature associated with the presence of a topically nontrivial electronic band structure in the vicinity of the Fermi level (EF). Through additional detailed theoretical analysis, we also found that an isostructural allotrope of the superconducting ${\delta}-$TaN phase, the simple hexagonal structure, ${\theta}-$TaN, has larger Berry curvature, and that, together with expected reasonable charge conductivity, it can also be a promising candidate for exploring a generation of spin-orbit torque magnetic random access memory as cheap, temperature stable, and highly efficient spin current sources.",2207.08872v2 2023-03-30,Observation of non-superconducting phase changes in LuH$_{2\pm\text{x}}$N$_y$,"The recent report of near-ambient superconductivity in nitrogen doped lutetium hydride has triggered a worldwide fanaticism and raised major questions about the latest claims. An intriguing phenomenon of color changes in pressurized samples from blue to pink to red was observed and correlated with the claimed superconducting transition, but the origin and underlying physics of these color changes have yet to be elucidated. Here we report synthesis and characterization of high-purity nitrogen doped lutetium hydride LuH$_{2\pm\text{x}}$N$_y$ with the same structure and composition as in the main phase of near-ambient superconductor1. We find a new purple phase of LuH$_{2\pm\text{x}}$N$_y$ between blue and pink phase, and reveal that the sample color changes likely stem from pressure-driven redistribution of nitrogen and its interaction with the LuH$_2$ framework. No superconducting transition is found in all blue, purple, pink and red phases at temperatures 1.8-300 K and pressures 0-30 GPa. Instead, we identify a notable temperature-induced resistance anomaly of structural and/or electronic origin in LuH$_{2\pm\text{x}}$N$_y$, which is most pronounced in the pink phase and may have been erroneously interpreted as a sign of superconducting transition. This work establishes key benchmarks for nitrogen doped lutetium hydrides, allowing an in-depth understanding of the novel pressure-induced phase changes.",2303.17587v2 2023-10-02,Resistless EUV lithography: photon-induced oxide patterning on silicon,"In this work, we show the feasibility of extreme ultraviolet (EUV) patterning on an HF-treated Si(100) surface in the absence of a photoresist. EUV lithography is the leading lithography technique in semiconductor manufacturing due to its high resolution and throughput, but future progress in resolution can be hampered because of the inherent limitations of the resists. We show that EUV photons can induce surface reactions on a partially H-terminated Si surface and assist the growth of an oxide layer, which serves as an etch mask. This mechanism is different from the H-desorption in scanning tunneling microscopy-based lithography. We achieve SiO2/Si gratings with 75 nm half-pitch and 31 nm height, demonstrating the efficacy of the method and the feasibility of patterning with EUV lithography without the use of a photoresist. Further development of the resistless EUV lithography method can be a viable approach to nm-scale lithography by overcoming the inherent resolution and roughness limitations of photoresist materials.",2310.01268v1 2023-10-31,Signature of Topological Semimetal in Harmonic-honeycomb ReO3,"Transition-metal honeycomb compounds are capturing scientific attention due to their distinctive electronic configurations, underscored by the triangular-lattice spin-orbit coupling and competition between multiple interactions, paving the way for potential manifestations of phenomena such as Dirac semimetal, superconductivity, and quantum spin liquid states. These compounds can undergo discernible pressure-induced alterations in their crystallographic and electronic paradigms, as exemplified by our high-pressure (HP) synthesis and exploration of the honeycomb polymorph of ReO3 (P6322). This HP-P6322 polymorph bears a phase transition from P6322 to P63/mmc upon cooling around Tp = 250 K, as evidenced by the evolution of temperature-dependent magnetization (M-T curves), cell dimension, and conductivity initiated by an inherent bifurcation of the oxygen position in the ab plane. Insightful analysis of its band structure positions suggests this HP-P6322 polymorph being a plausible candidate for Dirac semimetal properties. This phase transition evokes anomalies in the temperature-dependent variation of paramagnetism (non-linearity) and a crossover from semiconductor to temperature-independent metal, showing a temperature independent conductivity behavior below ~200 K. Under increasing external pressure, both the Tp and resistance of this HP-polymorph is slightly magnetic-field dependent and undergo a ""V""-style evolution (decreasing and then increasing) before becoming pressure independent up to 20.2 GPa. Theoretical calculations pinpoint this anionic disorder as a probable catalyst for the decrement in the conductive efficiency and muted temperature-dependent conductivity response.",2310.20341v2 2024-01-13,Reliable operation of Cr$_2$O$_3$:Mg/ $β$-Ga$_2$O$_3$ p-n heterojunction diodes at 600$^\circ$C,"$\beta$-Ga$_2$O$_3$-based semiconductor heterojunctions have recently demonstrated improved performance at high voltages and elevated temperatures and are thus promising for applications in power electronic devices and harsh-environment sensors. However, the long-term reliability of these ultra-wide band gap (UWBG) semiconductor devices remains barely addressed and may be strongly influenced by chemical reactions at the p-n heterojunction interface. Here, we experimentally demonstrate operation and evaluate the reliability of Cr$_2$O$_3$:Mg/ $\beta$-Ga$_2$O$_3$ p-n heterojunction diodes at during extended operation at 600$^\circ$C, as well as after 30 repeated cycles between 25-550$^\circ$C. The calculated pO2-temperature phase stability diagram of the Ga-Cr-O material system predicts that Ga$_2$O$_3$ and Cr$_2$O$_3$ should remain thermodynamically stable in contact with each other over a wide range of oxygen pressures and operating temperatures. The fabricated Cr$_2$O$_3$:Mg / $\beta$-Ga$_2$O$_3$ p-n heterojunction diodes show room-temperature on/off ratios >10$^4$ at $\pm$5V and a breakdown voltage (V$_{Br}$) of -390V. The leakage current increases with increasing temperature up to 600$^\circ$C, which is attributed to Poole-Frenkel emission with a trap barrier height of 0.19 eV. Over the course of a 140-hour thermal soak at 600$^\circ$C, both the device turn-on voltage and on-state resistance increase from 1.08V and 5.34 m$\Omega$-cm$^2$ to 1.59V and 7.1 m$\Omega$-cm$^2$ respectively. This increase is attributed to the accumulation of Mg and MgO at the Cr$_2$O$_3$/Ga$_2$O$_3$ interface as observed from TOF-SIMS analysis. These findings inform future design strategies of UWBG semiconductor devices for harsh environment operation and underscore the need for further reliability assessments for $\beta$-Ga$_2$O$_3$ based devices.",2401.07166v1 2024-02-09,BaMn$_2$P$_2$: Highest magnetic ordering temperature 122-pnictide compound,"We report the growth of high-quality single crystals of ThCr$_2$Si$_2$-type tetragonal BaMn$_2$P$_2$ and investigation of its structural, electrical transport, thermal and magnetic properties. Our results of basal plane electrical resistivity and heat capacity measurements show that the compound has an insulating ground state with a small band gap. Anisotropic susceptibility $\chi_{ab,c}(T)$ data infer a collinear local-moment N\'eel-type antiferromagnetic (AFM) ground state below the ordering temperature $T_{\rm N} = 795(15)$~K, which is highest among all the ThCr$_2$Si$_2$- and CaAl$_2$Si$_2$-type 122-pnictide compounds reported so far suggesting that the strength of magnetic exchange interactions is strongest in this material. The magnetic transition temperatures of BaMn$_2$$Pn_{2}$ ($Pn$ = P, As, Sb, Bi) compounds exhibit a monotonic decrease with the increase of tetragonal unit cell parameters $a$ and $c$, suggesting a strong dependence of the strength of the decisive magnetic exchange interactions on the separation between the localized spins residing on the Mn-ions. The observed monotonic increase of both $\chi_{ab}$ and $\chi_{c}$ for $T > T_{\rm N}$ suggests that short-range dynamic quasi-two dimensional AFM correlations persist above the $T_{\rm N}$ up to the highest temperature of the measurements. The large $T_{\rm N}$ of BaMn$_2$P$_2$ demands for systematic hole-doping studies on this material as similar investigations on related BaMn$_2$As$_{2}$ with $T_{\rm N} = 618$~K have led to the discovery of an outstanding ground state where AFM of localized Mn-spins and itinerant half-metallic ferromagnetism with $T_{\rm c} \approx 100$~K originating from the doped holes coexist together.",2402.06432v1 2016-07-07,Temperature dependence of the electrical resistivity and the anisotropic magnetoresistance (AMR) of electrodeposited Ni Co alloys,"The electrical resistivity and the anisotropic magnetoresistance (AMR) was investigated for Ni Co alloys at and below room temperature. The Ni Co alloy layers having a thickness of about 2 um were prepared by electrodeposition on Si wafers with evaporated Cr and Cu underlayers. The alloy composition was varied in the whole concentration range by varying the ratio of Ni sulfate and Co sulfate in the electrolyte. The Ni Co alloy deposits were investigated first in the as deposited state on the substrates and then, by mechanically stripping them from the substrates, as self supporting layers both without and after annealing. According to an X ray diffraction study, a strongly textured face centered cubic (fcc) structure was formed in the as deposited state with an average grain size of about 10 nm. Upon annealing, the crystal structure was retained whereas the grain size increased by a factor of 3 to 5, depending on alloy composition. The zero field resistivity decreased strongly by annealing due to the increased grain size. The annealing hardly changed the AMR below 50 at.% Co but strongly decreased it above this concentration. The composition dependence of the resistivity and the AMR of the annealed Ni Co alloy deposits was in good quantitative agreement with the available literature data both at 13 K and at room temperature. Both transport parameters were found to exhibit a pronounced maximum in the composition range between 20 and 30 at.% Co and the data of the Ni Co alloys fit well to the limiting values of the pure component metals (fcc Ni and fcc Co). The only theoretical calculation reported formerly on fcc Ni Co alloys yielded at T=0K a resistivity value smaller by a factor of 5 and an AMR value larger by a factor of about 2 than the corresponding low temperature experimental data, although the theoretical results properly reproduced the composition dependence of both quantities.",1607.01960v1 2012-06-07,Resistive and magnetoresistive properties of CrO2 pressed powders with different types of inter-granular dielectric layers,"Resistive, magnetoresistive and magnetic properties of four kinds of pressed CrO2 powders, synthesized by hydrothermal method of chromic anhydride have been investigated. The particles in powders constituted of rounded particles (diameter 120 nm) or needle-shaped crystals with an average diameter of 22.9 nm and average length of 302 nm. All of the particles had a surface dielectric shell of varying thickness and different types (such as oxyhydroxide -CrOOH or chromium oxide Cr2O3). For all the samples at low temperatures we found non-metallic temperature dependence of resistivity and giant negative magnetoresistance (MR). The maximum value of MR at low temperatures (T \approx 5 K) is \approx 37% in relatively small fields (0.5 T). At higher temperatures there was a rapid decrease of MR (up to \approx 1% / T at T \approx 200 K). The main objective of this work was studying the influence of properties and thickness of the intergranular dielectric layers, as well as CrO2 particle shape, on the magnitude of the tunneling resistance and MR of the pressed powder. The new results obtained in this study include: (1) detection at low temperatures in powders with needle-like particles a new type of MR hysteresis, and nonmonotonic MR behaviour with increasing magnetic field (absolute value of the MR at first grows rather rapidly with the field, and then begins diminishing markedly, forming a maximum), and (2) detection of non-monotonic temperature dependence, where - a field in which the resistance in a magnetic field has a maximum, as well as finding discrepancies in values of and coercivity fields, (3) detection of the anisotropy of MR, depending on the relative orientation of the transport current and the magnetic field, (4) a new method of synthesis, to regulate the thickness of dielectric coating.",1206.1533v1 2021-07-23,Modeling the dynamical behavior of memristive {NiTi} alloy at constant stress for time-varying electric current input signals,"The dynamical electric behavior of a NiTi smart alloy thin filament when driven by time varying current pulses is studied by a structure-based phenomenological model that includes rate-based effects. The simulation model relates the alloy's electrical resistivity to the relative proportions of the three main structural phases namely Martensite, Austenite and R-phase, experimentally known to exist in NiTi alloy lattice structure. The relative proportions of the phases depend on temperature and applied stress. Temperature varies due to the self-heating of the filament by the Joule effect when a current pulse passes and also due to convective/radiative interchange with the ambient. The temperature variation with time causes structural phase transitions, which result in abrupt changes in the sample resistivity as the proportions of each lattice phase vary. The model is described by a system of four 1st-order nonlinear differential-algebraic equations yielding the temporal evolution of resistivity and output voltage across the filament for any given time-varying input current pulse. The model corresponds to a 4th-order extended memristor, described by four state variables, which are the proportions of each of the three NiTi lattice phases and temperature. Simulations are experimentally verified by comparing to measurements obtained for samples self-heated by triangular current input waveforms as well as for passively samples with no current input. Numerical results reproduce very well measurements of resistance vs. temperature at equilibrium as well as the full dynamics of experimentally observed I-V characteristic curves and resistance vs. driving current for time-varying current input waveforms of a wide range of frequencies (0.01-10~Hz).",2107.11060v1 2024-05-06,Speckle pattern analysis of PVK:rGO composite based memristor device,"The memristors are expected to be fundamental devices for neuromorphic systems and switching applications. For example, the device made of a sandwiched layer of poly(N-vinylcarbazole) and reduced graphene composite between asymmetric electrodes (ITO/PVK:rGO/Al) exhibits bistable resistive switching behavior. Depending on the resistance state of the (ON-state or OFF-state) at a constant applied voltage, it may show two different resistivities. The performance of the memristor can be optimized by controlling the doping amount of graphene oxide in the PVK polymer. To assess the performance of the device, when it switches between ON and OFF states, optical characterization approaches are highly promising due to their non-destructive and remote nature. Here, we characterize the memristor device by the use of speckle pattern (SP) analysis. The speckle pattern is the interference of multiple light waves with random relative phases, which is generated via different mechanisms such as scattering from diffusive materials. Therefore, SPs can be used to investigate such samples as they include a huge amount of information to be statistically elaborated. The experimental paradigm includes \textit{in situ} acquisition of SPs of the PVK:rGO in different states followed by statistical post-processing toward examining its conduction mechanism. The variations in these statistical parameters are attributed to the resistance state of the PVK:rGO samples under the applied voltage with regard to the physical switching mechanism of the device. The resistance/conduction state, in turn, depends on the activity and properties of PVK:rGO memristors as well as the additional non-uniformities induced through the variations of density of carriers. The present optical methodology can be potentially served as a bench-top device for characterization purposes of similar devices while they are operating.",2405.03369v1 2017-10-09,Superconductivity in the Nb-Ru-Ge $σ$-Phase,"We show that the previously unreported ternary $\sigma$-phase material Nb$_{20.4}$Ru$_{5.7}$Ge$_{3.9}$ is a superconductor with a critical temperature of 2.2 K. Temperature-dependent magnetic susceptibility, resistance, and specific heat measurements were used to characterize the superconducting transition. The Sommerfeld constant $\gamma$ for Nb$_{20.4}$Ru$_{5.7}$Ge$_{3.9}$ is 91 mJ mol-f.u.$^{-1}$K$^{-2}$ and the specific heat anomaly at the superconducting transition, $\Delta$C/$\gamma$T$_c$, is approximately 1.38. The zero-temperature upper critical field ($\mu_0$H$_{c2}$(0)) was estimated to be 2 T by resistance data. Field-dependent magnetization data analysis estimated $\mu_0$H$_{c1}$(0) to be 5.5 mT. Thus, the characterization shows Nb$_{20.4}$Ru$_{5.7}$Ge$_{3.9}$ to be a type II BCS superconductor. This material appears to be the first reported ternary phase in the Nb-Ru-Ge system, and the fact that there are no previously reported binary Nb-Ru, Nb-Ge, or Ru-Ge $\sigma$-phases shows that all three elements are necessary to stabilize the material. A $\sigma$-phase in the Ta-Ru-Ge system was synthesized but did not display superconductivity above 1.7 K, which suggests that electron count cannot govern the superconductivity observed. Preliminary characterization of a possible superconducting $\sigma$-phase in the Nb-Ru-Ga system is also reported.",1710.03347v1 2022-02-28,Colloquium: Quantum anomalous Hall effect,"The quantum Hall (QH) effect, quantized Hall resistance combined with zero longitudinal resistance, is the characteristic experimental fingerprint of Chern insulators - topologically non-trivial states of two-dimensional matter with broken time-reversal symmetry. In Chern insulators, non-trivial bulk band topology is expressed by chiral states that carry current along sample edges without dissipation. The quantum anomalous Hall (QAH) effect refers to QH effects that occur in the absence of external magnetic fields due to spontaneously broken time-reversal symmetry. The QAH effect has now been realized in four different classes of two-dimensional materials: (i) thin films of magnetically (Cr- and/or V-) doped topological insulators in the (Bi,Sb)2Te3 family, (ii) thin films of the intrinsic magnetic topological insulator MnBi2Te4, (iii) moir\'e materials formed from graphene, and (iv ) moir\'e materials formed from transition metal dichalcogenides. In this Article, we review the physical mechanisms responsible for each class of QAH insulator, highlighting both differences and commonalities, and comment on potential applications of the QAH effect.",2202.13902v4 2018-08-12,Low Temperature Specific Heat of Doped SrTiO$_3$: Doping Dependence of the Effective Mass and Kadowaki-Woods Scaling Violation,"We report wide-doping-range ($8 \times 10^{17}$ to $4 \times 10^{20}$ cm$^{-3}$ Hall electron density) low temperature specific heat measurements on single crystal SrTiO$_3$:Nb, correlated with electronic transport data and tight-binding modeling. Lattice dynamic contributions to specific heat are shown to be well understood, albeit with unusual sensitivity to doping, likely related to the behavior of soft modes. Electronic contributions to specific heat provide effective masses that increase substantially, from $1.8$ to $4.8 m_e$, across the two SrTiO$_3$ Lifshitz transitions. It is shown that this behavior can be quantitatively reconciled with quantum oscillation data and calculated band structure, establishing a remarkably doping-independent mass enhancement factor of $2.0$. Most importantly, with the doping-dependent $T^2$ resistivity prefactor and Sommerfeld coefficient known, Kadowaki-Woods scaling has been tested over the entire doping range probed. Despite classic Fermi liquid behavior in electronic specific heat, standard Kadowaki-Woods scaling is dramatically violated, highlighting the need for new theoretical descriptions of $T^2$ resistivity in SrTiO$_3$.",1808.03909v2 2015-06-07,Temperature dependent three-dimensional anisotropy of the magnetoresistance in WTe$_2$,"Extremely large magnetoresistance (XMR) was recently discovered in WTe$_2$, triggering extensive research on this material regarding the XMR origin. Since WTe$_2$ is a layered compound with metal layers sandwiched between adjacent insulating chalcogenide layers, this material has been considered to be electronically two-dimensional (2D). Here we report two new findings on WTe$_2$: (1) WTe$_2$ is electronically 3D with a mass anisotropy as low as $2$, as revealed by the 3D scaling behavior of the resistance $R(H,\theta)=R(\varepsilon_\theta H)$ with $\varepsilon_\theta =(\cos^2 \theta + \gamma^{-2}\sin^2 \theta)^{1/2}$, $\theta$ being the magnetic field angle with respect to c-axis of the crystal and $\gamma$ being the mass anisotropy; (2) the mass anisotropy $\gamma$ varies with temperature and follows the magnetoresistance behavior of the Fermi liquid state. Our results not only provide a general scaling approach for the anisotropic magnetoresistance but also are crucial for correctly understanding the electronic properties of WTe$_2$, including the origin of the remarkable 'turn-on' behavior in the resistance versus temperature curve, which has been widely observed in many materials and assumed to be a metal-insulator transition.",1506.02214v2 2019-10-09,Preferential out-of-plane conduction and quasi-one-dimensional electronic states in layered 1T-TaS2,"Layered transition metal dichalcogenides (TMDs) are commonly classified as quasi-two-dimensional materials, meaning that their electronic structure closely resembles that of an individual layer, which results in resistivity anisotropies reaching thousands. Here, we show that this rule does not hold for 1T-TaS2 - a compound with the richest phase diagram among TMDs. While the onset of charge density wave order makes the in-plane conduction non-metallic, we reveal that the out-of-plane charge transport is metallic and the resistivity anisotropy is close to one. We support our findings with ab-initio calculations predicting a pronounced quasi-one-dimensional character of the electronic structure. Consequently, we interpret the highly debated metal-insulator transition in 1T-TaS2 as a quasi-one-dimensional instability, contrary to the long-standing Mott localisation picture. In a broader context, these findings are relevant for the newly born field of van der Waals heterostructures, where tuning interlayer interactions (e.g. by twist, strain, intercalation, etc.) leads to new emergent phenomena.",1910.03817v2 2019-10-23,Complex Transport and Magnetism in Inhomogeneous Mixed Valence Ce$_3$Ir$_4$Ge$_{13}$,"We report the discovery of Ce$_3$Ir$_4$Ge$_{13}$, a new Remeika phase compound with a complex array of structural, electronic, and magnetic properties. Our single crystal x-ray diffraction measurements show that Ce$_3$Ir$_4$Ge$_{13}$ forms in the tetragonally distorted $I4_1/amd$ space group. The electrical resistivity is almost temperature independent over three decades in temperature, from 0.4 K to 400 K, while the Hall coefficient measurements are consistent with a low-carrier semimetal. Magnetic susceptibility measurements reveal an effective moment of $\mu^{\text{exp}}_{\text{eff}} = 1.87 \mu_B$/Ce, suggesting that this material has a mixture of magnetic Ce$^{3+}$ and non-magnetic Ce$^{4+}$. Upon cooling, Ce$_3$Ir$_4$Ge$_{13}$ first enters a short range magnetically ordered state below $T_{\text{SRO}}=10$ K, marked by a deviation from Curie-Weiss behavior in susceptibility and a broad field-independent heat capacity anomaly. At lower temperatures, we observe a second, sharper peak in the heat capacity at $T^* = 1.7$ K, concurrent with a splitting of the field-cooled and zero-field-cooled susceptibilities. A small resistivity drop at $T^*$ suggests a loss of spin disorder scattering consistent with a magnetic ordering or spin freezing transition. Ce$_3$Ir$_4$Ge$_{13}$ is therefore a rare example of an inhomogeneous mixed valence compound with a complex array of thermodynamic and transport properties.",1910.10764v1 2020-05-01,Characterisation of Cryogenic Material Properties of 3D-Printed Superconducting Niobium using a 3D Lumped Element Microwave Cavity,"We present an experimental characterisation of the electrical properties of 3D-printed Niobium. The study was performed by inserting a 3D-printed Nb post inside an Aluminium cylindrical cavity, forming a 3D lumped element re-entrant microwave cavity resonator. The resonator was cooled to temperatures below the critical temperature of Niobium (9.25K) and then Aluminium (1.2K), while measuring the quality factors of the electromagnetic resonances. This was then compared with finite element analysis of the cavity and a measurement of the same cavity with an Aluminium post of similar dimensions and frequency, to extract the surface resistance of the Niobium post. The 3D-printed Niobium exhibited a transition to the superconducting state at a similar temperature to the regular Niobium, as well as a surface resistance of $3.1\times10^{-4}$ $\Omega$. This value was comparable to many samples of traditionally machined Niobium previously studied without specialised surface treatment. Furthermore, this study demonstrates a simple new method for characterizing the material properties of a relatively small and geometrically simple sample of superconductor, which could be easily applied to other materials, particularly 3D-printed materials. Further research and development in additive manufacturing may see the application of 3D-printed Niobium in not only superconducting cavity designs, but in the innovative technology of the future.",2005.00271v1 2021-09-30,Spin-flip-driven giant magneto-transport in A-type antiferromagnet NaCrTe2,"For anisotropic magneto-resistance (AMR) effect, its value synergistically depends on the magnitudes of magneto-resistance (MR) and magneto-crystalline anisotropy energy (MAE) simultaneously. In a magnetic material, the concurrence of gigantic AMR and MR signals is rather difficult due to weak spin-lattice coupling and small MAE. Here we report the considerable magneto-transport effect in layered A-type antiferromagnetic (AFM) NaCrTe2 by realigning the spin configurations. By applying H, the antiparallel spins of adjacent layers are flipped to ferromagnetic (FM) coupling either Ising-type along c-axis or XY-type within ab-plane. Theoretical calculations reveal that the energy bandgap narrows from 0.39 eV to 0.11 eV, accompanying a transition from semiconductor (high-R state) and half-semiconductor (low-R state), respectively. Thus, gigantic negative MR ratio of -90% is obtained at 10 K. More importantly, the decrement of R along H//c is far quicker than that of H//ab because the MAE of Ising-FM state is 1017 {\mu}eV/Cr3+ lower than that of XY-FM. The distinct trends result in the AMR ratio of 732% at 10 K, which is the record value to our best knowledge. These findings unravel the intrinsic origin of magneto in NaCrTe2 and will stimulate us to exploring the H-sensitive transport property in more AFM materials.",2109.14923v1 2021-11-12,Recrystallization and Interdiffusion Processes in Laser-Annealed Strain-Relaxed Metastable Ge$_{0.89}$Sn0$_{.11}$,"The prospect of GeSn semiconductors for silicon-integrated infrared optoelectronics brings new challenges related to the metastability of this class of materials. As a matter of fact, maintaining a reduced thermal budget throughout all processing steps of GeSn devices is essential to avoid possible material degradation. This constraint is exacerbated by the need for higher Sn contents along with an enhanced strain relaxation to achieve efficient mid-infrared devices. Herein, as a low thermal budget solution for post-epitaxy processing, we elucidate the effects of laser thermal annealing (LTA) on strain-relaxed Ge$_{0.89}$Sn0$_{.11}$ layers and Ni-Ge$_{0.89}$Sn0$_{.11}$ contacts. Key diffusion and recrystallization processes are proposed and discussed in the light of systematic microstructural studies. LTA treatment at a fluence of 0.40 J/cm2 results in a 200-300 nm-thick layer where Sn atoms segregate toward the surface and in the formation of Sn-rich columnar structures in the LTA-affected region. These structures are reminiscent to those observed in the dislocation-assisted pipe-diffusion mechanism, while the buried GeSn layers remain intact. Moreover, by tailoring the LTA fluence, the contact resistance can be reduced without triggering phase separation across the whole GeSn multi-layer stacking. Indeed, a one order of magnitude decrease in the Ni-based specific contact resistance was obtained at the highest LTA fluence, thus confirming the potential of this method for the functionalization of direct bandgap GeSn materials.",2111.06788v1 2022-04-18,Material properties of a low contraction and resistivity silicon-aluminum composite for cryogenic detectors,"We report on the cryogenic properties of a low-contraction silicon-aluminum composite, namely Japan Fine Ceramics SA001, to use as a packaging structure for cryogenic silicon devices. SA001 is a silicon--aluminum composite material (75% silicon by volume) and has a low thermal expansion coefficient ($\sim$1/3 that of aluminum). The superconducting transition temperature of SA001 is measured to be 1.18 K, which is in agreement with that of pure aluminum, and is thus available as a superconducting magnetic shield material. The residual resistivity of SA001 is 0.065 $\mathrm{\mu \Omega m}$, which is considerably lower than an equivalent silicon--aluminum composite material. The measured thermal contraction of SA001 immersed in liquid nitrogen is $\frac{L_{293\mathrm{K}}-L_{77\mathrm{K}}}{L_{293\mathrm{K}}}=0.12$%, which is consistent with the expected rate obtained from the volume-weighted mean of the contractions of silicon and aluminum. The machinability of SA001 is also confirmed with a demonstrated fabrication of a conical feedhorn array, with a wall thickness of 100 $\mathrm{\mu m}$. These properties are suitable for packaging applications for large-format superconducting detector devices.",2204.08111v2 2022-06-07,Phase-field modelling and analysis of rate-dependent fracture phenomena at finite deformation,"Fracture of materials with rate-dependent mechanical behaviour, e.g. polymers, is a highly complex process. For an adequate modelling, the coupling between rate-dependent stiffness, dissipative mechanisms present in the bulk material and crack driving force has to be accounted for in an appropriate manner. In addition, the fracture toughness, i.e. the resistance against crack propagation, can depend on rate of deformation. In this contribution, an energetic phase-field model of rate-dependent fracture at finite deformation is presented. For the deformation of the bulk material, a formulation of finite viscoelasticity is adopted with strain energy densities of Ogden type assumed. The unified formulation allows to study different expressions for the fracture driving force. Furthermore, a possibly rate-dependent toughness is incorporated. The model is calibrated using experimental results from the literature for an elastomer and predictions are qualitatively and quantitatively validated against experimental data. Predictive capabilities of the model are studied for monotonic loads as well as creep fracture. Symmetrical and asymmetrical crack patterns are discussed and the influence of a dissipative fracture driving force contribution is analysed. It is shown that, different from ductile fracture of metals, such a driving force is not required for an adequate simulation of experimentally observable crack paths and is not favourable for the description of failure in viscoelastic rubbery polymers. Furthermore, the influence of a rate-dependent toughness is discussed by means of a numerical study. From a phenomenological point of view, it is demonstrated that rate-dependency of resistance against crack propagation can be an essential ingredient for the model when specific effects such as rate-dependent brittle-to-ductile transitions shall be described.",2206.03460v1 2022-11-17,On universal butterfly and antisymmetric magnetoresistances,"Butterfly magnetoresistance (BMR) and antisymmetric magnetoresistance (ASMR) are about a butterfly-cross curve and a curve with one peak and one valley when a magnetic field is swept up and down along a fixed direction. Other than the parallelogram-shaped magnetoresistance-curve (MR-curve) often observed in magnetic memory devices, BMR and ASMR are two ubiquitous types of MR-curves observed in diversified magnetic systems, including van der Waals materials, strongly correlated systems, and traditional magnets. Here, we reveal the general principles and the picture behind the BMR and the ASMR that do not depend on the detailed mechanisms of magnetoresistance: 1) The systems exhibit hysteresis loops, common for most magnetic materials with coercivities. 2) The magnetoresistance of the magnetic structures in a large positive magnetic field and in a large negative magnetic field is approximately the same. With the generalized Ohm's law in magnetic materials, these principles explain why most BMR appears in the longitudinal resistance measurements and is very rare in the Hall resistance measurements. Simple toy models, in which the Landau-Lifshitz-Gilbert equation governs magnetization, are used to demonstrate the principles and explain the appearance and disappearance of BMR in various experiments. Our finding provides a simple picture to understand magnetoresistance-related experiments.",2211.09369v1 2009-03-16,Interplay between magnetism and superconductivity and appearance of a second superconducting transition in alpha-FeSe at high pressure,"We synthesized tetragonal alpha-FeSe by melting a powder mixture of iron and selenium at high pressure. Subsequent annealing at normal pressure results in removing traces of hexagonal beta- FeSe, formation of a rather sharp transition to superconducting state at Tc ~ 7 K, and the appearance of a magnetic transition near Tm = 120 K. Resistivity and ac-susceptibility were measured on the annealed sample at hydrostatic pressure up to 4.5 GPa. A magnetic transition visible in ac-susceptibility shifts down under pressure and the resistive anomaly typical for a spin density wave (SDW) antiferromagnetic transition develops near the susceptibility anomaly. Tc determined by the appearance of a diamagnetic response in susceptibility, increases linearly under pressure at a rate dTc/dP = 3.5 K/GPa. Below 1.5 GPa, the resistive superconducting transition is sharp; the width of transition does not change with pressure; and, Tc determined by a peak in drho/dT increases at a rate ~ 3.5 K/GPa. At higher pressure, a giant broadening of the resistive transition develops. This effect cannot be explained by possible pressure gradients in the sample and is inherent to alpha-FeSe. The dependences drho(T)/dT show a signature for a second peak above 3 GPa which is indicative of the appearance of another superconducting state in alpha-FeSe at high pressure. We argue that this second superconducting phase coexists with SDW antiferromagnetism in a partial volume fraction and originates from pairing of charge carriers from other sheets of the Fermi surface.",0903.2873v1 2022-05-19,High pressure structural and magneto-transport studies on type-II Dirac semimetal candidate Ir2In8S: Emergence of superconductivity upon decompression,"The structural and magneto-transport properties of type-II Dirac semimetal candidate Ir2In8S have been investigated under high pressure. The ambient tetragonal structure (P4_2/mnm) is found to be stable up to 7 GPa, above which the system takes an orthorhombic Pnnm structure, possibly destroying the Dirac cones due to the loss of the four-fold screw symmetry. In the tetragonal structure, a gradual suppression of the transverse magneto-resistance and a rapid change in the magnetic field dependence above 50K suggest possible T-dependent Fermi surface modification. In the high pressure phase, the metallic character increases marginally (as evident from the increased RRR value) accompanied with suppressed magneto-resistance, without emergence of superconductivity up to 20 GPa and down to 1.4K. Most surprisingly, upon release of pressure to 0.2 GPa, a sharp resistance drop below 4K is observed, field varying measurements confirm this as the onset of superconductivity. The observed changes of the carrier density and mobility in the pressure-released tetragonal phase indicate electronic structural modification resulting from the irreversible polyhedral distortion. A simultaneous increase in the residual resistivity and carrier density upon decompression indicates that an enhanced impurity scattering play a key role in the emergence of superconductivity in the tetragonal Ir2In8S, making it an ideal platform to study topological superconductivity.",2205.09798v1 2022-11-08,Effective resistivity in relativistic collisionless plasmoid-mediated reconnection,"Magnetic reconnection can power spectacular high-energy astrophysical phenomena by producing non-thermal energy distributions in highly magnetized regions around compact objects. By means of two-dimensional fully kinetic particle-in-cell (PIC) simulations we investigate relativistic collisionless plasmoid-mediated reconnection in magnetically dominated pair plasmas with and without guide field. In X-points, where diverging flows result in a non-diagonal thermal pressure tensor, a finite residence time for particles gives rise to a localized collisionless effective resistivity. Here, for the first time for relativistic reconnection in a fully developed plasmoid chain we identify the mechanisms driving the non-ideal electric field using a full Ohm's law by means of a statistical analysis based on our PIC simulations. We show that the non-ideal electric field is predominantly driven by gradients of nongyrotropic thermal pressures. We propose a kinetic physics motivated non-uniform effective resistivity model, which is negligible on global scales and becomes significant only locally in X-points, that captures the properties of collisionless reconnection with the aim of mimicking its essentials in non-ideal magnetohydrodynamic descriptions. This effective resistivity model provides a viable opportunity to design physically grounded global models for reconnection-powered high-energy emission.",2211.04553v1 2023-10-23,Deep learning denoiser assisted roughness measurements extraction from thin resists with low Signal-to-Noise Ratio(SNR) SEM images: analysis with SMILE,"The technological advance of High Numerical Aperture Extreme Ultraviolet Lithography (High NA EUVL) has opened the gates to extensive researches on thinner photoresists (below 30nm), necessary for the industrial implementation of High NA EUVL. Consequently, images from Scanning Electron Microscopy (SEM) suffer from reduced imaging contrast and low Signal-to-Noise Ratio (SNR), impacting the measurement of unbiased Line Edge Roughness (uLER) and Line Width Roughness (uLWR). Thus, the aim of this work is to enhance the SNR of SEM images by using a Deep Learning denoiser and enable robust roughness extraction of the thin resist. For this study, we acquired SEM images of Line-Space (L/S) patterns with a Chemically Amplified Resist (CAR) with different thicknesses (15nm, 20nm, 25nm, 30nm), underlayers (Spin-On-Glass-SOG, Organic Underlayer-OUL) and frames of averaging (4, 8, 16, 32, and 64 Fr). After denoising, a systematic analysis has been carried out on both noisy and denoised images using an open-source metrology software, SMILE 2.3.2, for investigating mean CD, SNR improvement factor, biased and unbiased LWR/LER Power Spectral Density (PSD). Denoised images with lower number of frames present unaltered Critical Dimensions (CDs), enhanced SNR (especially for low number of integration frames), and accurate measurements of uLER and uLWR, with the same accuracy as for noisy images with a consistent higher number of frames. Therefore, images with a small number of integration frames and with SNR < 2 can be successfully denoised, and advantageously used in improving metrology throughput while maintaining reliable roughness measurements for the thin resist.",2310.14815v1 2023-04-13,Combining Electron-Phonon and Dynamical Mean-Field Theory Calculations of Correlated Materials: Transport in the Correlated Metal Sr$_2$RuO$_4$,"Electron-electron ($e$-$e$) and electron-phonon ($e$-ph) interactions are challenging to describe in correlated materials, where their joint effects govern unconventional transport, phase transitions, and superconductivity. Here we combine first-principles $e$-ph calculations with dynamical mean field theory (DMFT) as a step toward a unified description of $e$-$e$ and $e$-ph interactions in correlated materials. We compute the $e$-ph self-energy using the DMFT electron Green's function, and combine it with the $e$-$e$ self-energy from DMFT to obtain a Green's function including both interactions. This approach captures the renormalization of quasiparticle dispersion and spectral weight on equal footing. Using our method, we study the $e$-ph and $e$-$e$ contributions to the resistivity and spectral functions in the correlated metal Sr$_2$RuO$_4$. In this material, our results show that $e$-$e$ interactions dominate transport and spectral broadening in the temperature range we study (50$-$310~K), while $e$-ph interactions are relatively weak and account for only $\sim$10\% of the experimental resistivity. We also compute effective scattering rates, and find that the $e$-$e$ interactions result in scattering several times greater than the Planckian value $k_BT$, whereas $e$-ph interactions are associated with scattering rates lower than $k_BT$. Our work demonstrates a first-principles approach to combine electron dynamical correlations from DMFT with $e$-ph interactions in a consistent way, advancing quantitative studies of correlated materials.",2304.06771v2 2011-07-13,SDW transition of Fe1 zigzag chains and metamagnetic transition of Fe2 in TaFe$_{1+y}$Te$_3$,"We systematically study the AFM order of Fe1 zigzag chains and spin-flop of excess Fe2 under high magnetic field H through the susceptibility, magnetoresistance (MR), Hall effect and specific heat measurements in high-quality single crystal TaFe$_{1+y}$Te$_3$. These properties suggest that the high temperature AFM transition of the TaFeTe$_3$ layers should be a SDW-type AFM order. Below T$_N$, Fe1 antiferromangetic zigzag chains will induce a inner magnetic field \textbf{H$_{int}$} to interstitial Fe2 and lead Fe2 also forms an AFM alignment, in which the magnetic coupling strength between Fe1 and Fe2 is enhanced by decreasing temperature. On the other hand, the external magnetic field \textbf{H$_{ext}$} inclines to tune interstitial Fe2 to form FM alignment along \textbf{H$_{ext}$}. When \textbf{H$_{ext}$} arrives at the ""coercive"" field H$_C$, which is able to break the coupling between Fe1 and Fe2, these interstitial Fe2 atoms take a spin-flop from AFM to FM alignment. The local moment of Fe2 is about 4 $\mu_{\textrm{B}}$/Fe. From low field ($<$H$_C$) AFM to high field ($>$H$_C$) FM for Fe2, it also induces sharp drop on resistivity and an anomalous Hall effect. The possible magnetic structure of TaFe$_{1+y}$Te$_3$ is proposed from the susceptibility and MR. The properties related to the spin-flop of Fe2 supply a good opportunity to study the coupling between Fe1 and Fe2 in these TaFe$_{1+y}$Te$_3$ or Fe$_{1+y}$Te with interstitial Fe2 compounds.",1107.2561v1 2012-05-06,Free-Electron Laser-Powered Electron Paramagnetic Resonance Spectroscopy,"Electron paramagnetic resonance (EPR) spectroscopy interrogates unpaired electron spins in solids and liquids to reveal local structure and dynamics; for example, EPR has elucidated parts of the structure of protein complexes that have resisted all other techniques in structural biology. EPR can also probe the interplay of light and electricity in organic solar cells and light-emitting diodes, and the origin of decoherence in condensed matter, which is of fundamental importance to the development of quantum information processors. Like nuclear magnetic resonance (NMR), EPR spectroscopy becomes more powerful at high magnetic fields and frequencies, and with excitation by coherent pulses rather than continuous waves. However, the difficulty of generating sequences of powerful pulses at frequencies above 100 GHz has, until now, confined high-power pulsed EPR to magnetic fields of 3.5 T and below. Here we demonstrate that ~1 kW pulses from a free-electron laser (FEL) can power a pulsed EPR spectrometer at 240 GHz (8.5 T), providing transformative enhancements over the alternative, a state-of-the-art ~30 mW solid state source. Using the UC Santa Barbara FEL as a source, our 240 GHz spectrometer can rotate spin-1/2 electrons through pi/2 in only 6 ns (vs. 300 ns with the solid state source). Fourier transform EPR on nitrogen impurities in diamond demonstrates excitation and detection of EPR lines separated by ~200 MHz. Decoherence times for spin-1/2 systems as short as 63 ns are measured, enabling measurement of the decoherence time in a frozen solution of nitroxide free-radicals at temperatures as high as 190 K. Both FELs and the quasi-optical technology developed for the spectrometer are scalable to frequencies well in excess of 1 THz, opening the possibility of high-power pulsed EPR spectroscopy up to the highest static magnetic fields on earth.",1205.1186v1 2014-02-10,Development of CMOS pixel sensors for tracking and vertexing in high energy physics experiments,"CMOS pixel sensors (CPS) represent a novel technological approach to building charged particle detectors. CMOS processes allow to integrate a sensing volume and readout electronics in a single silicon die allowing to build sensors with a small pixel pitch ($\sim 20 \mu m$) and low material budget ($\sim 0.2-0.3\% X_0$) per layer. These characteristics make CPS an attractive option for vertexing and tracking systems of high energy physics experiments. Moreover, thanks to the mass production industrial CMOS processes used for the manufacturing of CPS the fabrication construction cost can be significantly reduced in comparison to more standard semiconductor technologies. However, the attainable performance level of the CPS in terms of radiation hardness and readout speed is mostly determined by the fabrication parameters of the CMOS processes available on the market rather than by the CPS intrinsic potential. The permanent evolution of commercial CMOS processes towards smaller feature sizes and high resistivity epitaxial layers leads to the better radiation hardness and allows the implementation of accelerated readout circuits. The TowerJazz $0.18 \mu m$ CMOS process being one of the most relevant examples recently became of interest for several future detector projects. The most imminent of these project is an upgrade of the Inner Tracking System (ITS) of the ALICE detector at LHC. It will be followed by the Micro-Vertex Detector (MVD) of the CBM experiment at FAIR. Other experiments like ILD consider CPS as one of the viable options for flavour tagging and tracking sub-systems.",1402.2172v1 2020-04-23,SENSEI: Direct-Detection Results on sub-GeV Dark Matter from a New Skipper-CCD,"We present the first direct-detection search for eV-to-GeV dark matter using a new ~2-gram high-resistivity Skipper-CCD from a dedicated fabrication batch that was optimized for dark-matter searches. Using 24 days of data acquired in the MINOS cavern at the Fermi National Accelerator Laboratory, we measure the lowest rates in silicon detectors of events containing one, two, three, or four electrons, and achieve world-leading sensitivity for a large range of sub-GeV dark matter masses. Data taken with different thicknesses of the detector shield suggest a correlation between the rate of high-energy tracks and the rate of single-electron events previously classified as ""dark current."" We detail key characteristics of the new Skipper-CCDs, which augur well for the planned construction of the ~100-gram SENSEI experiment at SNOLAB.",2004.11378v3 2018-12-04,Superconductivity at 250 K in lanthanum hydride under high pressures,"The discovery of superconductivity at 203 K in H3S brought attention back to conventional superconductors whose properties can be described by the Bardeen-Cooper-Schrieffer (BCS) and the Migdal-Eliashberg theories. These theories predict that high, and even room temperature superconductivity (RTSC) is possible in metals possessing certain favorable parameters such as lattice vibrations at high frequencies. However, these general theories do not suffice to predict real superconductors. New superconducting materials can be predicted now with the aid of first principles calculations based on Density Functional Theory (DFT). In particular, the calculations suggested a new family of hydrides possessing a clathrate structure, where the host atom (Ca, Y, La) is at the center of the cage formed by hydrogen atoms. For LaH10 and YH10 superconductivity, with critical temperatures Tc ranging between 240 and 320 K is predicted at megabar pressures. Here, we report superconductivity with a record Tc ~ 250 K within the Fm-3m structure of LaH10 at a pressure P ~ 170 GPa. We proved the existence of superconductivity at 250 K through the observation of zero-resistance, isotope effect, and the decrease of Tc under an external magnetic field, which suggests an upper critical magnetic field of 120 T at zero-temperature. The pressure dependence of the transition temperatures Tc (P) has a maximum of 250-252 K at the pressure of about 170 GPa. This leap, by ~ 50 K, from the previous Tc record of 203 K indicates the real possibility of achieving RTSC (that is at 273 K) in the near future at high pressures and the perspective of conventional superconductivity at ambient pressure.",1812.01561v1 2021-09-18,Microstructural engineering of medium entropy NiCo(CrAl) alloy for enhanced room and high-temperature mechanical properties,"This work demonstrates the development of a strong and ductile medium entropy alloy by employing conventional alloying and thermomechanical processing to induce partial recrystallization (PR) and precipitation strengthening in the microstructure. The combined usage of electron microscopy and atom probe tomography reveals the sequence of microstructural evolution during the process. First, the cold working of homogenized alloy resulted in a highly deformed microstructure. On annealing at 700{\deg}C, B2 ordered precipitates heterogeneously nucleate on the highly misoriented sites. These B2 promotes particle stimulated nucleation (PSN) of new recrystallized strain-free grains. The migration of recrystallized grain boundaries leads to discontinuous precipitation of L12 ordered regions in highly dense lamellae structures. Atomic-scale compositional analysis reveals a significant amount of Ni confined to the GB regions between B2 and L12 precipitates, indicating Ni as a rate-controlling element for coarsening the microstructure. On 20 hours of annealing, the alloy comprises a composite microstructure of soft recrystallized and hard non-recrystallized zones, B2 particles at the grain boundaries (GBs), and coherent L12 precipitates inside the grains. The B2 pins the GB movement during recrystallization while the latter provides high strength. The microstructure results in a 0.2% yield stress (YS) value of 1030 MPa with 32% elongation at ambient temperature and retains up to 910 MPa at 670{\deg}C. Also, it shows exceptional microstructural stability at 700 {\deg}C and resistance to deformation at high temperatures up to 770{\deg}C. Examination of deformed microstructure reveals excessive twinning, formation of stacking faults, shearing of L12 precipitates, and accumulation of dislocations at around the B2 precipitates and GBs attributed to high strain hardening of the alloy.",2109.08894v3 2022-10-07,Fast time-domain current measurement for quantum dot charge sensing using a homemade cryogenic transimpedance amplifier,"We developed a high-speed and low-noise time-domain current measurement scheme using a homemade GaAs high-electron-mobility-transistor-based cryogenic transimpedance amplifier (TIA). The scheme is versatile for broad cryogenic current measurements, including semiconductor spin-qubit readout, owing to the TIA's having low input impedance comparable to that of commercial room-temperature TIAs. The TIA has a broad frequency bandwidth and a low noise floor, with a trade-off between them governed by the feedback resistance $R_{FB}$. A lower $R_{FB}$ of 50 k$\Omega$ enables high-speed current measurement with a -3dB cutoff frequency $f_{-3dB}$ = 28 MHz and noise-floor $NF = 8.5 \times 10^{-27}$ A$^{2}$/Hz, while a larger $R_{FB}$ of 400 k$\Omega$ provides low-noise measurement with $NF = 1.0 \times 10^{-27}$ A$^{2}$/Hz and $f_{-3dB}$ = 4.5 MHz. Time-domain measurement of a 2-nA peak-to-peak square wave, which mimics the output of the standard spin-qubit readout technique via charge sensing, demonstrates a signal-to-noise ratio (SNR) of 12.7, with the time resolution of 48 ns, for $R_{FB}$ = 200 k$\Omega$, which compares favorably with the best-reported values for the radio-frequency (RF) reflectometry technique. The time resolution can be further improved at the cost of the SNR (or vice versa) by using an even smaller (larger) $R_{FB}$, with a further reduction in the noise figure possible by limiting the frequency band with a low-pass filter. Our scheme is best suited for readout electronics for cryogenic sensors that require a high time resolution and current sensitivity and thus provides a solution for various fundamental research and industrial applications.",2210.03333v1 2001-03-20,Fully dense MgB_2 superconductor textured by hot deformation,"Bulk textured MgB_2 material of nearly full density showing a weak c-axis alignment of the hexagonal MgB_2 grains parallel to the pressure direction was obtained by hot deformation of a stoichiometric MgB_2 pellet prepared by a gas-solid reaction. The texture of the material was verified by comparing the x-ray diffraction patterns of the hot deformed material with isotropic MgB_2 powder. A small, but distinct anisotropy of the upper critical field up to Hc2^{a,b}/Hc2^{c}~1.2 depending on degree of texture was found by resistance and susceptibility measurements. No anisotropy of the critical current density determined from magnetization measurements was found for the textured material.",0103408v2 2004-11-22,Quantized Failure Criteria and Indirect Observation for Predicting the Nanoscale Strength of Materials: The Example of the Ultra Nano Crystalline Diamond,"In this paper theoretical and statistical/experimental criteria for determining the nanoscale strength of materials are proposed. In particular, quantized criteria in fracture mechanics, dynamic fracture mechanics and fatigue, as well as an experimental indirect observation of the nanoscale strength, are proposed. The increasing of the dynamic resistance and the role of a fractal crack surface formation are also rationalized. The analysis shows that materials can be sensitive to flaws also at nanoscale (as demonstrated for carbon nanotubes), in contrast to the conclusion of a recently published paper, and that the surfaces are weaker than the inner parts of a solid by a factor of about 10%. In addition, the proposed statistical/experimental procedure is applied for predicting the nanoscale strength of the ultrananocrystalline diamond (UNCD), an innovative material only recently developed.",0411556v1 2010-08-05,Evaluation of the acoustic and non-acoustic properties of sound absorbing materials using a three-microphone impedance tube,"This paper presents a straightforward application of an indirect method based on a three-microphone impedance tube setup to determine the non-acoustic properties of a sound absorbing porous material. First, a three-microphone impedance tube technique is used to measure some acoustic properties of the material (i.e., sound absorption coefficient, sound transmission loss, effective density and effective bulk modulus) regarded here as an equivalent fluid. Second, an indirect characterization allows one to extract its non-acoustic properties (i.e., static airflow resistivity, tortuosity, viscous and thermal characteristic lengths) from the measured effective properties and the material open porosity. The procedure is applied to four different sound absorbing materials and results of the characterization are compared with existing direct and inverse methods. Predictions of the acoustic behavior using an equivalent fluid model and the found non-acoustic properties are in good agreement with impedance tube measurements.",1008.0975v1 2011-02-20,Intrinsic Correlation between Hardness and Elasticity in Polycrystalline Materials and Bulk Metallic Glasses,"Though extensively studied, hardness, defined as the resistance of a material to deformation, still remains a challenging issue for a formal theoretical description due to its inherent mechanical complexity. The widely applied Teter's empirical correlation between hardness and shear modulus has been considered to be not always valid for a large variety of materials. Here, inspired by the classical work on Pugh's modulus ratio, we develop a theoretical model which establishes a robust correlation between hardness and elasticity for a wide class of materials, including bulk metallic glasses, with results in very good agreement with experiment. The simplified form of our model also provides an unambiguous theoretical evidence for Teter's empirical correlation.",1102.4063v1 2014-07-05,Large-scale BN tunnel barriers for graphene spintronics,"We have fabricated graphene spin-valve devices utilizing scalable materials made from chemical vapor deposition (CVD). Both the spin-transporting graphene and the tunnel barrier material are CVD-grown. The tunnel barrier is realized by h-BN, used either as a monolayer or bilayer and placed over the graphene. Spin transport experiments were performed using ferromagnetic contacts deposited onto the barrier. We find that spin injection is still greatly suppressed in devices with a monolayer tunneling barrier due to resistance mismatch. This is, however, not the case for devices with bilayer barriers. For those devices, a spin relaxation time of 260 ps intrinsic to the CVD graphene material is deduced. This time scale is comparable to those reported for exfoliated graphene, suggesting that this CVD approach is promising for spintronic applications which require scalable materials.",1407.1439v1 2017-02-16,Large elastic recovery of zinc dicyanoaurate,"We report the mechanical properties of the `giant' negative compressibility material zinc(II) dicyanoaurate, as determined using a combination of single-crystal nanoindentation measurements and \emph{ab initio} density functional theory calculations. While the elastic response of zinc dicyanoaurate is found to be intermediate to the behaviour of dense and open framework structures, we discover the material to exhibit a particularly strong elastic recovery, which is advantageous for a range of practical applications. We attribute this response to the existence of supramolecular helices that function as atomic-scale springs, storing mechanical energy during compressive stress and hence inhibiting plastic deformation. Our results are consistent with the relationship noted in [Cheng \& Cheng, \textit{Appl. Phys. Lett.}, 1998, {\textbf{73}}, 614] between the magnitude of elastic recovery, on the one hand, and the ratio of material hardness to Young's modulus, on the other hand. Drawing on comparisons with other metal--organic frameworks containing helical structure motifs, we suggest helices as an attractive supramolecular motif for imparting resistance to plastic deformation in the design of functional materials.",1702.05145v1 2018-06-19,Hydrodynamic Phonon Transport Perpendicular to Diffuse-Gray Boundaries,"In this paper, we examine the application of an ideal phonon-hydrodynamic material as the heat transfer medium between two non-hydrodynamic contacts with a finite temperature difference. We use the integral-equation approach to solve a modified phonon Boltzmann transport equation with the displaced Bose-Einstein distribution as the equilibrium distribution between two boundaries perpendicular to the heat transfer direction. When the distance between the boundaries is smaller than the phonon normal scattering mean free path, our solution converges to the ballistic limit as expected. In the other limit, we find that, although the local thermal conductivity in the bulk of the hydrodynamic material approaches infinity, the thermal boundary resistance at the hydrodynamic/non-hydrodynamic interfaces becomes dominant. Our study provides insights to both the steady-state thermal characterization of phonon-hydrodynamic materials and the practical application of phonon-hydrodynamic materials for thermal management.",1806.07345v3 2019-08-26,One-pot synthesis: a simple and fast method to obtain ceramic superconducting materials,"The one-pot method focuses on the reduction of the number of steps or chemical reactions in the synthesis of materials, and it is very appealing in terms of sustainability. In addition to this point of view, superconductors are desired materials due to their unusual properties, such as the zero resistivity and the perfect diamagnetism. One-pot, Thus, in this work, we described the one-pot synthesis of YBa2Cu3O7-{\delta} superconducting ceramic. In just two steps and a few hours, a polymer composite solution was prepared, which originates a powder after burning the polymer out with pure phase and with superconducting properties better than those produced by other techniques.",1908.09923v1 2018-07-16,Tailoring Materials for Mottronics: Excess Oxygen Doping of a Prototypical Mott Insulator,"The Mott transistor is a paradigm for a new class of electronic devices---often referred to by the term Mottronics---, which are based on charge correlations between the electrons. Since correlation-induced insulating phases of most oxide compounds are usually very robust, new methods have to be developed to push such materials right to the boundary to the metallic phase in order to enable the metal-insulator transition to be switched by electric gating. Here we demonstrate that thin films of the prototypical Mott insulator LaTiO$_3$ grown by pulsed laser deposition under oxygen atmosphere are readily tuned by excess oxygen doping across the line of the band-filling controlled Mott transition in the electronic phase diagram. The detected insulator to metal transition is characterized by a strong change in resistivity of several orders of magnitude. The use of suitable substrates and capping layers to inhibit oxygen diffusion facilitates full control of the oxygen content and renders the films stable against exposure to ambient conditions, making LaTiO$_{3+x}$ a promising functional material for Mottronics devices.",1807.05724v1 2020-11-25,Reconstructing the thermal phonon transmission coefficient at solid interfaces in the phonon transport equation,"The ab initio model for heat propagation is the phonon transport equation, a Boltzmann-like kinetic equation. When two materials are put side by side, the heat that propagates from one material to the other experiences thermal boundary resistance. Mathematically, it is represented by the reflection coefficient of the phonon transport equation on the interface of the two materials. This coefficient takes different values at different phonon frequencies, between different materials. In experiments scientists measure the surface temperature of one material to infer the reflection coefficient as a function of phonon frequency. In this article, we formulate this inverse problem in an optimization framework and apply the stochastic gradient descent (SGD) method for finding the optimal solution. We furthermore prove the maximum principle and show the Lipschitz continuity of the Fr\'echet derivative. These properties allow us to justify the application of SGD in this setup.",2011.13047v2 2023-01-24,Using Arduino in Physics Experiments:Determining the Speed of Sound in Air,"Considering the 21st century skills and the importance of STEM education in fulfilling these skills, it is clear that the course materials should be materials that bring students together with technology and attract their attention, apart from traditional materials. In addition, in terms of the applicability of these materials, it is very important that the materials are affordable and easily accessible. In this study two open ended resonance tube, Computer and speaker for generate sound with different frequencies, Arduino UNO, AR-054 Sound Sensor, Green LED and 220 ohm resistance were used for measure the speed of sound in air at room tempature. With the help of sound sensor, two consecutive harmonic frequency values were determined and the fundamental frequency was calculated. Using the tube features and the fundamental frequency value, the speed of sound propagation in the air at room temperature was calculated as 386.42 m/s. This value is theoretically 346 m/s. This study, in which the propagation speed of the sound is calculated with very low cost and coding studies with 12% error margin, is important in terms of hosting all STEM gains and can be easily applied in classrooms.",2301.10325v1 2023-09-14,Photo-induced reversible modification of the Curie-Weiss temperature in paramagnetic gadolinium compounds,"Gadolinium oxyhydride GdHO is a photochromic material that darkens under illumination and bleaches back by thermal relaxation. As an inorganic photochromic material that can be easily deposited by magnetron sputtering, GdHO has very interesting potential applications as a functional material, specially for smart glazing applications. However, the underlying reasons behind the photochromic mechanism-which can be instrumental for the correct optimisation of GdOH for different applications-are not completely understood. In this paper, we rely on the well-stablished magnetic properties of Gd$^{3+}$ to shed light on this matter. GdOH thin films present paramagnetic behaviour similar to other Gd$^{3+}$ compounds such as Gd$_2$O$_3$. Illumination of the films result in a reversible increase of the Curie-Weiss temperature pointing to RKKY interactions, which is consistent with the resistivity decrease observed in the photo-darkened films.",2309.07978v1 2024-01-26,First-principles Methodology for studying magnetotransport in magnetic materials,"Unusual magnetotransport behaviors such as temperature dependent negative magnetoresistance(MR) and bowtie-shaped MR have puzzled us for a long time. Although several mechanisms have been proposed to explain them, the absence of comprehensive quantitative calculations has made these explanations less convincing. In our work, we introduce a methodology to study the magnetotransport behaviors in magnetic materials. This approach integrates anomalous Hall conductivity induced by Berry curvature, with a multi-band ordinary conductivity tensor, employing a combination of first-principles calculations and semi-classical Boltzmann transport theory. Our method incorporates both the temperature dependency of relaxation time and anomalous Hall conductivity, as well as the field dependency of anomalous Hall conductivity. We initially test this approach on two-band models and then apply it to a Weyl semimetal \CSS. The results, which align well with experimental observations in terms of magnetic field and temperature dependencies, demonstrate the efficacy of our approach. Additionally, we have investigated the distinct behaviors of magnetoresistance (MR) and Hall resistivities across various types of magnetic materials. This methodology provides a comprehensive and efficient means to understand the underlying mechanisms of the unusual behaviors observed in magneto-transport measurements in magnetic materials.",2401.15146v1 2024-03-29,Computational Shape Derivatives in Heat Conduction: An Optimization Approach for Enhanced Thermal Performance,"We analyze an optimization problem of the conductivity in a composite material arising in a heat conduction energy storage problem. The model is described by the heat equation that specifies the heat exchange between two types of materials with different conductive properties with Dirichlet-Neumann boundary conditions on the external part of the domain, and on the interface characterized by the resisting coefficient between the highly conductive material and the less conductive material. The main purpose of the paper is to compute a shape gradient of an optimization functional in order to accurately determine the optimal location of the conductive material using a classical shape optimization strategy. We also present some numerical experiments to illustrate the efficiency of the proposed method.",2403.20181v1 2002-05-30,Tunability of High-Dielectric-Constant Materials from First Principles,"A first-principles method, based on density functional perturbation theory, is presented for computing the leading order tunability of high-dielectric-constant materials.",0205655v1 2024-05-28,On the resistance regular graphs,"For a connected graph $G$, its resistance matrix is denoted by $R(G)$. If all the row(column) sums of $R(G)$ are equal, then $G$ is said to be resistance regular. In $[13]$, J. Zhou et al. posed the question regarding the existence of a non-regular resistance regular graph. In this article, we establish that all resistance regular graphs are regular, thus conclusively answering Zhou's question by showing that no non-regular resistance regular graph exists. Also, we compute the resistance energies of some resistance regular graphs. Furthermore, we determine various bounds for the resistance energy and resistance spectral radius of $G.$",2405.18177v1 2005-06-29,Galaxy formation and cosmic-ray acceleration in a magnetized universe,"We study the linear magneto-hydrodynamical behaviour of a Newtonian cosmology with a viscous magnetized fluid of finite conductivity and generalise the Jeans instability criterion. The presence of the field favors the anisotropic collapse of the fluid, which in turn leads to further magnetic amplification and to an enhanced current-sheet formation in the plane normal to the ambient magnetic field. When the currents exceed a certain threshold, the resulting electrostatic turbulence can dramatically amplify the resistivity of the medium (anomalous resistivity). This could trigger strong electric fields and subsequently the acceleration of ultra-high energy cosmic rays (UHECRs) during the formation of protogalactic structures.",0506742v1 1998-10-21,Large scale instabilities in two-dimensional magnetohydrodynamics,"The stability of a sheared magnetic field is analyzed in two-dimensional magnetohydrodynamics with resistive and viscous dissipation. Using a multiple-scale analysis, it is shown that at large enough Reynolds numbers the basic state describing a motionless fluid and a layered magnetic field, becomes unstable with respect to large scale perturbations. The exact expressions for eddy-viscosity and eddy-resistivity are derived in the nearby of the critical point where the instability sets in. In this marginally unstable case the nonlinear phase of perturbation growth obeys to a Cahn-Hilliard-like dynamics characterized by coalescence of magnetic islands leading to a final new equilibrium state. High resolution numerical simulations confirm quantitatively the predictions of multiscale analysis.",9810026v1 1997-11-19,Intrinsic resistivity and the SO(5) theory of high-temperature superconductors,"The topological structure of the order parameter in Zhang's SO(5) theory of superconductivity allows for an unusual type of dissipation mechanism via which current-carrying states can decay. The resistivity due to this mechanism, which involves orientation rather than amplitude order-parameter fluctuations, is calculated for the case of a thin superconducting wire. The approach is a suitably modified version of that pioneered by Langer and Ambegaokar for conventional superconductors.",9711193v2 1998-05-22,reentrance effect in normal-metal/superconducting hybrid loops,"We have measured the transport properties of two mesoscopic hybrid loops composed of a normal-metal arm and a superconducting arm. The samples differed in the transmittance of the normal/superconducting interfaces. While the low transmittance sample showed monotonic behavior in the low temperature resistance, magnetoresistance and differential resistance, the high transmittance sample showed reentrant behavior in all three measurements. This reentrant behavior is due to coherent Andreev reflection at the normal/superconducting interfaces. We compare the reentrance effect for the three different measurements and discuss the results based on the theory of quasiclassical Green's functions.",9805298v1 1998-12-20,"Comment on ""Charged impurity scattering limited low temperature resistivity of low density silicon inversion layers"" (Das Sarma and Hwang, cond-mat/9812216)","In a recent preprint cond-mat/9812216, Das Sarma and Hwang propose an explanation of the sharp decrease in resistivity at low temperatures which has been attributed to a transition to an unexpected conducting phase in dilute high-mobility two-dimensional systems at B=0. In this Comment, we examine whether their model is supported by the available experimental data.",9812331v1 1999-02-24,Charge Relaxation and Dephasing in Coulomb Coupled Conductors,"The dephasing time in coupled mesoscopic conductors is caused by the fluctuations of the dipolar charge permitted by the long range Coulomb interaction. We relate the phase breaking time to elementary transport coefficients which describe the dynamics of this dipole: the capacitance, an equilibrium charge relaxation resistance and in the presence of transport through one of the conductors a non-equilibrium charge relaxation resistance. The discussion is illustrated for a quantum point contact in a high magnetic field in proximity to a quantum dot.",9902320v1 1999-03-31,Apparent Metallic Behavior at B = 0 of a two-dimensional electron system in AlAs,"We report the observation of metallic-like behavior at low temperatures and zero magnetic field in two dimensional (2D) electrons in an AlAs quantum well. At high densities the resistance of the sample decreases with decreasing temperature, but as the density is reduced the behavior changes to insulating, with the resistance increasing as the temperature is decreased. The effect is similar to that observed in 2D electrons in Si-MOSFETs, and in 2D holes in SiGe and GaAs, and points to the generality of this phenomenon.",9903443v1 1999-04-05,Spin Degree of Freedom in a Two-Dimensional Electron Liquid,"We have investigated correlation between spin polarization and magnetotransport in a high mobility silicon inversion layer which shows the metal-insulator transition. Increase in the resistivity in a parallel magnetic field reaches saturation at the critical field for the full polarization evaluated from an analysis of low-field Shubnikov-de Haas oscillations. By rotating the sample at various total strength of the magnetic field, we found that the normal component of the magnetic field at minima in the diagonal resistivity increases linearly with the concentration of ``spin-up'' electrons.",9904058v1 1999-06-17,Systematic Evolution of the Magnetotransport Properties of Bi_{2}Sr_{2-x}La_{x}CuO_{6} with Carrier Concentration,"We report that it is possible to obtain a series of high-quality crystals of La-doped Bi-2201, of which the transport properties have been believed to be ""dirtier"" than those of other cuprates. In our crystals, the normal-state transport properties display behaviors which are in good accord with other cuprates; for example, in the underdoped region the in-plane resistivity \rho_{ab} shows the pseudogap feature and in the overdoped region the T dependence of \rho_{ab} changes to T^n with n > 1. The characteristic temperatures of the pseudogap deduced from the resistivity and the Hall coefficient data are presented.",9906268v1 2000-02-08,Negative Pressure of Anisotropic Compressible Hall States : Implication to Metrology,"Pressure, compressibility, and Hall conductance of anisotropic states at higher Landau levels are computed. Pressure and compressibility become negative. Hall conductance is unquantized and varies with filling factor. These facts agree with the recent experimental observations of highly anisotropic compressible states at higher Landau levels. It is shown, as an implication of negative pressure, that the quantum Hall effect has extraordinary stability, that is, Hall resistance is quantized even when the longitudinal resistance does not vanish.",0002108v3 2000-12-08,"Pressure, Resistance, and Current Activation of Anisotropic Compressible Hall States","Thermodynamic and electric properties of anisotropic compressible Hall states at higher Landau levels are studied using a mean field theory on the von Neumann lattice basis. It is shown that resistances agree with the recent experiments of anisotropic compressible states and the states have negative pressure. As implications, the collapse phenomena of the integer quantum Hall effect are discussed.",0012133v1 2001-07-03,Scaling Behavior of Anomalous Hall Effect and Longitudinal Nonlinear Response in High-Tc Superconductors,"Based on existing theoretical model and by considering our longitudinal nonlinear response function, we derive a nonliear equation in which the mixed state Hall resistivity can be expressed as an analytical function of magnetic field, temperature and applied current. This equation enables one to compare quantitatively the experimental data with theoretical model. We also find some new scaling relations of the temperature and field dependency of Hall resistivity. The comparison between our theoretical curves and experimental data shows a fair agreement.",0107045v1 2001-07-06,"Current-Driven Conformational Changes, Charging and Negative Differential Resistance in Molecular Wires","We introduce a theoretical approach based on scattering theory and total energy methods that treats transport non-linearities, conformational changes and charging effects in molecular wires in a unified way. We apply this approach to molecular wires consisting of chain molecules with different electronic and structural properties bonded to metal contacts. We show that non-linear transport in all of these systems can be understood in terms of a single physical mechanism and predict that negative differential resistance at high bias should be a generic property of such molecular wires.",0107147v1 2001-07-17,Analysis of the resistance in p-SiGe over a wide temperature range,"The temperature dependence of a system exhibiting a `metal-insulator transition in two dimensions at zero magnetic field' (MIT) is studied up to 90K. Using a classical scattering model we are able to simulate the non-monotonic temperature dependence of the resistivity in the metallic high density regime. We show that the temperature dependence arises from a complex interplay of metallic and insulating contributions contained in the calculation of the scattering rate $1/\td(E,T)$, each dominating in a limited temperature range.",0107369v1 2001-09-27,Enhanced paramagnetism of the 4d itinerant electrons in the rhodium oxide perovskite SrRhO3,"Polycrystalline rhodium(IV) oxide perovskite SrRhO3 was obtained by high-pressure synthesis techniques, followed by measurements of the magnetic susceptibility, electrical resistivity, and specific heat. The title compound has five 4d-electrons per perovskite unit and shows Fermi-liquid behavior in its electrical resistivity. The magnetic susceptibility is large [chi(300K) \~1.1*10^{-3} emu/mol-Rh] and proportional to 1/T^2 (< 380 K), while there is no magnetic long-range order above 1.8 K. The specific heat measurements indicate a probable magnetic contribution below ~ 15 K, which is not predicted by the self-consistent renormalization theory of spin fluctuations for both antiferro- and ferromagnetic 3D nearly-ordered metals.",0109522v2 2001-12-20,Fluctuation induced hopping and spin polaron transport,"We study the motion of free magnetic polarons in a paramagnetic background of fluctuating local moments. The polaron can tunnel only to nearby regions of local moments when these fluctuate into alignment. We propose this fluctuation induced hopping as a new transport mechanism for the spin polaron. We calculate the diffusion constant for fluctuation induced hopping from the rate at which local moments fluctuate into alignment. The electrical resistivity is then obtained via the Einstein relation. We suggest that the proposed transport mechanism is relevant in the high temperature phase of the Mn pyrochlore colossal magneto resistance compounds and Europium hexaboride.",0112385v1 2002-11-27,Indications of coherence-incoherence crossover in layered transport,"For many layered metals the temperature dependence of the interlayer resistance has a different behavior than the intralayer resistance. In order to better understand interlayer transport we consider a concrete model which exhibits this behavior. A small polaron model is used to illustrate how the interlayer transport is related to the coherence of quasi-particles within the layers. Explicit results are given for the electron spectral function, interlayer optical conductivity and the interlayer magnetoresistance. All these quantities have two contributions: one coherent (dominant at low temperatures) and one incoherent (dominant at high temperatures).",0211612v1 2002-11-28,Small polarons and c-axis transport in highly anisotropic metals,"Motivated by the anomalous c-axis transport properties of the quasi two-dimensional metal, $\rm Sr_2 Ru O_4$, and related compounds, we have studied the interlayer hopping of single electrons that are coupled strongly to c-axis bosons. We find a c-axis resistivity that reflects the in-plane electronic scattering in the low and very high temperature limits (relative to the characteristic temperature of the boson $T_{\rm boson}$). For temperatures near the $T_{\rm boson}$, a broad maximum in the resistivity can appear for sufficiently strong electron-boson coupling. This feature may account for the observed ``metallic to non-metallic crossover'' seen in these layered oxides, where the boson may be a phonon.",0211675v1 2003-05-01,Negative differential resistance due to the resonance coupling of a quantum-dot dimer,"Electron tunneling through a coupled quantum-dot dimer under a dc-bias is investigated. We find that a peak in the $I$-$V$ curve appears at low temperature when two discrete electronic states in the two quantum dots are aligned with each other -- resonance coupling. This leads to a negative differential resistance. The peak height and width depend on the dot-dot coupling. At high temperature, the peak disappears due to thermal smearing effects.",0305018v1 2003-08-06,Measuring thermal conductivity in extreme conditions: sub-Kelvin temperatures and high (27 T) magnetic fields,"We present a one-heater-two-thermometer set-up for measuring thermal conductivity and electric resistivity of a bulk sample at low temperatures down to 0.1 K and in magnetic fields up to 27 Tesla. The design overcomes the difficulties emerging in the context of large water-cooled resistive magnets.",0308106v1 2003-09-29,Fluxon dynamics by microwave surface resistance measurements in MgB2,"Field-induced variations of the microwave surface resistance, Rs(H), have been investigated in high-density ceramic MgB2. At low temperatures, several peculiarities of the Rs(H) curves cannot be justified in the framework of models reported in the literature. We suggest that they are ascribable to the unconventional vortex structure in MgB2, related to the presence of two gaps. On the contrary, the results near Tc can be accounted for by the Coffey and Clem model, with fluxons moving in the flux-flow regime, provided that the anisotropy of the upper critical field is taken into due account.",0309654v1 2003-10-20,Evidence for a quantum phase transition in the electron-doped cuprate Pr2-xCexCuO4+d from Hall and resistivity measurements,"The doping and temperature dependence of the Hall coefficient, RH, and ab-plane resistivity in the normal state down to 350mK is reported for oriented films of the electron-doped high-Tc superconductor Pr2-xCexCuO4+d. The doping dependence of b (r=r0+AT^b) and R_sub_H (at 350 mK) suggest a quantum phase transition at a critical doping near x=0.165.",0310475v2 2004-01-15,Plasmon assisted transport through disordered array of quantum wires,"Phononless plasmon assisted thermally activated transport through a long disordered array of finite length quantum wires is investigated analytically. Generically strong electron plasmon interaction in quantum wires results in a qualitative change of the temperature dependence of thermally activated resistance in comparison to phonon assisted transport. At high temperatures, the thermally activated resistance is determined by the Luttinger liquid interaction parameter of the wires.",0401274v2 2004-01-26,Vanishing Hall Resistance at High Magnetic Field in a Double Layer Two-Dimensional Electron System,"At total Landau level filling factor $\nu_{tot}=1$ a double layer two-dimensional electron system with small interlayer separation supports a collective state possessing spontaneous interlayer phase coherence. This state exhibits the quantized Hall effect when equal electrical currents flow in parallel through the two layers. In contrast, if the currents in the two layers are equal, but oppositely directed, both the longitudinal and Hall resistances of each layer vanish in the low temperature limit. This finding supports the prediction that the ground state at $\nu_{tot}=1$ is an excitonic superfluid.",0401521v1 2004-07-06,Spin characterization and control over the regime of radiation-induced zero-resistance states,"Over the regime of the radiation-induced zero-resistance states and associated oscillatory magnetoresistance, we propose a low magnetic field analog of quantum-Hall-limit techniques for the electrical detection of electron spin- and nuclear magnetic- resonance, dynamical nuclear polarization via electron spin resonance, and electrical characterization of the nuclear spin polarization via the Overhauser shift. In addition, beats observed in the radiation-induced oscillatory-magnetoresistance are developed into a method to measure and control the zero-field spin splitting due to the Bychkov-Rashba and bulk inversion asymmetry terms in the high mobility GaAs/AlGaAs system.",0407143v1 2004-08-03,Electrical resistivity and tunneling anomalies in CeCuAs2,"The compound CeCuAs2 is found to exhibit negative temperature (T) coefficient of electrical resistivity (rho) under ambient pressure conditions in the entire T-range of investigation (45 mK to 300 K), even in the presence of high magnetic fields. Preliminary tunneling spectroscopic measurements indicate the existence of a psuedo-gap at least at low temperatures, thereby implying that this compound could be classified as a Kondo semi-conductor, though rho(T) interestingly is not found to be of an activated type.",0408060v1 2005-01-05,Radiation-induced zero-resistance states with resolved Landau levels,"The microwave-photoexcited high mobility GaAs/AlGaAs two-dimensional electron system exhibits an oscillatory-magnetoresistance with vanishing resistance in the vicinity of magnetic fields $B = [4/(4j+1)] B_{f}$, where $B_{f} = 2\pi\textit{f}m^{*}/e$, m$^{*}$ is an the effective mass, e is the charge, \textit{f} is the microwave frequency, and $j$ =1,2,3... Here, we report transport with well-resolved Landau levels, and some transmission characteristics.",0501091v1 2005-01-21,Metallic behavior in Si/SiGe 2D electron systems,"We calculate the temperature, density, and parallel magnetic field dependence of low temperature electronic resistivity in 2D high-mobility Si/SiGe quantum structures, assuming the conductivity limiting mechanism to be carrier scattering by screened random charged Coulombic impurity centers. We obtain comprehensive agreement with existing experimental transport data, compellingly establishing that the observed 2D metallic behavior in low-density Si/SiGe systems arises from the peculiar nature of 2D screening of long-range impurity disorder. In particular, our theory correctly predicts the experimentally observed metallic temperature dependence of 2D resistivity in the fully spin-polarized system.",0501531v1 2005-05-10,Variable resistance at the boundary between semimetal and excitonic insulator,"We solve the two-band model for the transport across a junction between a semimetal and an excitonic insulator. We analyze the current in terms of two competing terms associated with neutral excitons and charged carriers, respectively. We find a high value for the interface resistance, extremely sensitive to the junction transparency. We explore favorable systems for experimental confirmation.",0505247v1 2006-02-18,Anomalous Flux Pinning in ?-Pyrochlore Oxide Superconductor KOs2O6,"The superconducting transition of the ?-pyrochlore oxide KOs2O6 with Tc = 9.60 K is studied by resistivity measurements under various magnetic fields using a high-quality single crystal. The reentrant behavior of superconductivity is observed near Tc in low magnetic fields below 2 T. The recovered resistance probably due to flux flow exhibits an anomalous angle dependence, indicating that flux pinning is enhanced in magnetic fields along certain crystallographic directions such as [110], [001] and [112]. It is suggested that there is an intrinsic pinning mechanism coming from the specific crystal structure of the ?-pyrochlore oxide.",0602433v1 2006-03-30,Joule heating induced negative differential resistance in free standing metallic carbon nanotubes,"The features of the $IV$ characteristics of metallic carbon nanotubes (m-NTs) in different experimental setups are studied using semi-classical Boltzmann transport equation together with the heat dissipation equation to account for significant thermal effects at high electric bias. Our model predicts that the shape of the m-NT characteristics is basically controlled by heat removal mechanisms. In particular we show that the onset of negative differential resistance in free standing nanotubes finds its origins in strong transport nonlinearities associated with poor heat removal unlike in substrate-supported nanotubes.",0603831v1 2007-03-27,Resistively shunted Josephson junctions: QFT predictions versus MC results,"During the last fourteen years several exact results were obtained for the so-called boundary sine-Gordon model. In the case of a conformal bulk this 2D boundary quantum field theory describes the universal scaling behavior of the Caldeira-Leggett model of resistively shunted Josephson junctions. In this work, we use a recently developed Monte Carlo technique to test some of the analytical predictions.",0703712v2 1994-02-14,Fractal Dimension of Gauge-fixing Defects,"The fractal dimension $D_f$ of sites resisting Landau or maximal Abelian(MA) gauge fixing in lattice $SU(3)$ gluodynamics is defined and computed. In Landau gauge such sites clump into $D_f\sim 1$ clusters in the confining phase. In the finite temperature phase their dimensionality drops to $D_f < 1$, that is, clustering seems to dissipate. In contrast, MA gauge resistant sites fail to exhibit a notable tendency to cluster at any temperature.",9402009v2 2002-07-09,Body Motion in a Resistive Medium at Temperature T,"We consider a macroscopic body propagating in a one-dimensional resistive medium, consisting of an ideal gas at temperature $T$. For a whole family of collisions with varying degree of inelasticity, we find an exact expression for the effective force on the moving body as a function of the body's speed and the value of the restitution coefficient. At low and high speeds it reduces to the well-known Stoke's and Newton's law, respectively.",0207037v1 2002-11-29,Resistive plate chambers for time-of-flight measurements,"The applications of Resistive Plate Chambers (RPCs) have recently been extended by the development of counters with time resolution below 100 ps sigma for minimum ionising particles. Applications to HEP experiments have already taken place and many further applications are under study. In this work we address the operating principles of such counters along with some present challenges, with emphasis on counter aging.",0211120v1 2007-05-04,Simultaneous recording of two- and four-probe resistive transitions in doped laser-processed Sr-Ru-O,"To confirm previously reported evidence of high-temperature superconductivity in laser processed Sr-Ru-O, we performed simultaneous two-probe and four-probe resistive measurements using bar-geometry samples. A superconducting-type transition with an onset at about 250K was recorded in one of the samples, consistent with our previously reported measurements in the X-bridge geometry. Some compositional details of the samples are also provided which were not known at the time of previous web-publication.",0705.0641v1 2007-07-18,"Synchnonization, zero-resistance states and rotating Wigner crystal","We show that rotational angles of electrons moving in two dimensions (2D) in a perpendicular magnetic field can be synchronized by an external microwave field which frequency is close to the Larmor frequency. The synchronization eliminates collisions between electrons and thus creates a regime with zero diffusion corresponding to the zero-resistance states observed in experiments with high mobility 2D electron gas (2DEG). For long range Coulomb interactions electrons form a rotating hexagonal Wigner crystal. Possible relevance of this effect for planetary rings is discussed.",0707.2694v1 2007-11-06,Plasmon phenomena as origin of DC-current induced resistivity oscillations in two-dimensional electron systems,"We analyze theoretically the oscillations that the magnetoresistivity of two-dimensional electron systems present when a high intensity direct current is applied. In the model presented here we suggest that a plasma wave is excited in the system producing an oscillating motion of the whole two-dimensional electron gas at the plasma frequency. This scenario affects dramatically the way that electrons interact with scatterers giving rise to oscillations in the longitudinal resistivity. With this theoretical model experimental results are well reproduced and explained.",0711.0927v1 2008-06-17,Electrical Resistivity and Specific Heat of EuFe2As2 Single Crystals: Magnetic homologue of SrFe2As2,"We have grown single crystals of EuFe2As2 and investigated its electrical transport and thermodynamic properties. Electrical resistivity and specific heat measurements clearly establish the intrinsic nature of magnetic phase transitions at 20 K and 195 K. While the high temperature phase transition is associated with the itinerant moment of Fe, the low temperature phase transition is due to magnetic order of localized Eu-moments. Band structure calculations point out a very close similarity of the electronic structure with SrFe2As2. Magnetically, the Eu and Fe2As2 sublattice are nearly de-coupled.",0806.2876v2 2008-08-05,Suppression of Magnetic Order by Pressure in BaFe2As2,"We performed the dc resistivity and the ZF 75As-NMR measurement of BaFe2As2 under high pressure. The T-P phase diagram of BaFe2As2 determined from resistivity anomalies and the ZF 75As-NMR clearly revealed that the SDW anomaly is quite robust against P.",0808.0718v1 2008-10-14,Magnetic Field Induced Instabilities in Localised Two-Dimensional Electron Systems,"We report density dependent instabilities in the localised regime of mesoscopic two-dimensional electron systems (2DES) with intermediate strength of background disorder. They are manifested by strong resistance oscillations induced by high perpendicular magnetic fields B_{\perp}. While the amplitude of the oscillations is strongly enhanced with increasing B_{\perp}, their position in density remains unaffected. The observation is accompanied by an unusual behaviour of the temperature dependence of resistance and activation energies. We suggest the interplay between a strongly interacting electron phase and the background disorder as a possible explanation.",0810.2418v1 2009-08-02,Resistivity noise in crystalline magnetic nanowires and its implications to domain formation and kinetics,"We have investigated the time-dependent fluctuations in electrical resistance, or noise, in high quality crystalline magnetic nanowires within nanoporous templates. The noise increases exponentially with increasing temperature and magnetic field, and has been analyzed in terms of domain wall depinning within the Neel-Brown framework. The frequency-dependence of noise also indicates a crossover from nondiffusive kinetics to long-range diffusion at higher temperatures, as well as a strong collective depinning, which need to be considered when implementing these nanowires in magnetoelectronic devices.",0908.0136v1 2010-07-07,Selfoscillations of Suspended Carbon Nanotubes with a Deflection Sensitive Resistance under Voltage Bias,"We theoretically investigate the electro-mechanics of a Suspended Carbon Nanotube with a Deflection Sensitive Resistance subjected to a homogeneous Magnetic Field and a constant Voltage Bias. We show that, (with the exception of a singular case), for a sufficiently high magnetic field the time-independent state of charge transport through the nanotube becomes unstable to selfexcitations of the mechanical vibration accompanied by oscialltions in the voltage drop and current across the nanotube.",1007.1139v1 2010-07-28,Inelastic contribution of the resistivity in the hidden order in URu2Si2,"In the hidden order of URu2Si2 the resistivity at very low temperature shows no T^2 behavior above the transition to superconductivity. However, when entering the antiferromagnetic phase, the Fermi liquid behavior is recovered. We discuss the change of the inelastic term when entering the AF phase with pressure considering the temperature dependence of the Grueneisen parameter at ambient pressure and the influence of superconductivity by an extrapolation of high field data.",1007.4905v1 2010-08-23,Field induced changes across magnetic compensation in Pr(1-x)Gd(x)Al(2) alloys,"The magnetic compensation phenomenon has been explored in the Pr(1-x)Gd(x)Al(2) series. The contributions from Pr and Gd moments compensate each other at a specific temperature in the ordered state (below (T(c)). At high fields, the magnetic reorientation (with respect to the external field direction) of the Pr and Gd moments appears as a minimum in the thermomagnetic response. We demonstrate several interesting attributes related with the magnetic reorienation phenomenon, viz., oscillatory behavior of the magneto-resistance, sign change of the anamalous Hall resistivity, fingerprints of field induced changes in the specific heat and ac-susceptibility data.",1008.3782v1 2011-01-14,Hall field-induced resistance oscillations in tilted magnetic fields,"We have studied the effect of an in-plane magnetic field on Hall field-induced resistance oscillations in high mobility two-dimensional electron systems. We have found that the oscillation frequency depends only on the perpendicular component of the magnetic field but the oscillation amplitude decays exponentially with an in-plane component. While these findings cannot be accounted for by existing theories of nonlinear transport, our analysis suggests that the decay can be explained by an in-plane magnetic field-induced modification of the quantum scattering rate.",1101.2871v2 2011-02-24,Positive speed for high-degree automaton groups,"Mother groups are the basic building blocks for polynomial automaton groups. We show that, in contrast with mother groups of degree 0 or 1, any bounded, symmetric, generating random walk on the mother groups of degree at least 3 has positive speed. The proof is based on an analysis of resistance in fractal mother graphs. We give upper bounds on resistances in these graphs, and show that infinite versions are tran- sient.",1102.4979v1 2011-03-09,An efficient multi-use multi-secret sharing scheme based on hash function,"In this paper, a renewable, multi-use, multi-secret sharing scheme for general access structure based on one-way collision resistant hash function is presented in which each participant has to carry only one share. By applying collision-resistant one-way hash function, the proposed scheme is secure against conspiracy attacks even if the pseudo-secret shares are compromised. Moreover, high complexity operations like modular multiplication, exponentiation and inversion are avoided to increase its efficiency. Finally, in the proposed scheme, both the combiner and the participants can verify the correctness of the information exchanged among themselves.",1103.1730v1 2011-05-28,Thermo-Resistive Instability in Magnetar Crusts,"We investigate a thermo-resistive instability in the outer crusts of magnetars wherein a perturbation in temperature increases ohmic heating. We show that magnetars of characteristic age {\tau}_{age} ~ 10^4 yr are unstable over timescales as short as days if strong current sheets are present in the outer crust. This instability could play an important role in the thermal and magnetic field evolution of magnetars, and may be related to bursting activity in magnetars.",1105.5712v1 2011-10-10,Non linear transport in drift-diffusion equations under magnetic field,"We analyze numerically and analytically the non linear transport properties of a drift-diffusion equation in presence of a magnetic field and of a disorder potential. For a wide range of parameters this model exhibits a plateau where the drift velocity is almost independent on the applied electric field. This behavior has strong similarities with the zero differential resistance states observed experimentally in high mobility two dimensional systems. Performed numerical simulations are in a good global agreement with the developed analytical theory even if the later leads to overestimated negative differential resistance values.",1110.2033v1 2012-08-09,Strange metals at finite 't Hooft coupling,"In this paper, we consider the AdS-Schwarzshild black hole in light-cone coordinates which exhibits non-relativistic z=2 Schrodinger symmetry. Then, we use the $AdS/CFT$ correspondence to investigate the effect of finite-coupling corrections to two important properties of the strange metals which are the Ohmic resistivity and the inverse Hall angle. It is shown that the Ohmic resistivity and inverse Hall angle are linear and quadratic temperature dependent in the case of $\mathcal{R}^4$ corrections, respectively. While in the case of Gauss-Bonnet gravity, we find that the inverse Hall angle is quadratic temperature dependent and the Ohmic conductivity can never be linear temperature dependent.",1208.1855v1 2012-11-15,Microwave-induced resistance oscillations in tilted magnetic fields,"We have studied the effect of an in-plane magnetic field on microwave-induced resistance oscillations in a high mobility two-dimensional electron system. We have found that the oscillation amplitude decays exponentially with an in-plane component of the magnetic field $B_\parallel$. While these findings cannot be accounted for by existing theories, our analysis suggests that the decay can be explained by a $B_\parallel$-induced correction to the quantum scattering rate, which is quadratic in $B_\parallel$.",1211.3753v1 2013-07-25,"Negative differential resistance with graphene channels, interfacing distributed quantum dots in Field-Effect Transistors","Field effect transistors with channels made of graphene layer(s) were explored. The graphene layer(s) contacted a distributed array of well-separated semiconductor quantum dots (QDs). The dots were embedded in nano-structured hole-array; each filled hole was occupied by one dot. Differential optical and electrical conductance was observed. Since Negative Differential Resistance (NDR) is key to high-speed elements, such construction may open the door for new electro-photonic devices.",1307.6790v1 2013-09-04,Exploiting negative differential resistance in monolayer graphene FETs for high voltage gains,"Through self-consistent quantum transport simulations, we evaluate the RF performance of monolayer graphene FETs in the bias region of negative output differential resistance. We show that, compared to the region of quasi-saturation, a voltage gain larger than 10 can be obtained, at the cost of a decrease in the maximum oscillation frequency of about a factor of 1.5--3 and the need for a careful circuit stabilization.",1309.1105v2 2013-11-01,Fermi liquid breakdown and evidence for superconductivity in YFe$_2$Ge$_2$,"In the d-electron system YFe$_2$Ge$_2$, an unusually high and temperature dependent Sommerfeld ratio of the specific heat capacity $C/T \sim 100~\mathrm{mJ/(molK^2)}$ and an anomalous power law temperature dependence of the electrical resistivity $\rho \simeq \rho_0 + AT^{3/2}$ signal Fermi liquid breakdown, probably connected to a close-by quantum critical point. Full resistive transitions, accompanied by DC diamagnetic screening fractions of up to 80\% suggest that pure samples of YFe$_2$Ge$_2$ superconduct below $1.8~\mathrm{K}$.",1311.0247v2 2014-04-28,Resistive Plate Chambers for Imaging Calorimetry - the DHCAL,"The DHCAL, the Digital Hadron Calorimeter, is a prototype calorimeter based on Resistive Plate Chambers (RPCs). The design emphasizes the imaging capabilities of the detector in an effort to optimize the calorimeter for the application of Particle Flow Algorithms (PFAs) to the reconstruction of hadronic jet energies in a colliding beam environment. The readout of the chambers is segmented into 1 x 1 cm2 pads, each read out with a 1-bit (single threshold) resolution. The prototype with approximately 500,000 readout channels underwent extensive testing in both the Fermilab and CERN test beams. This talk presents preliminary findings from the analysis of data collected at the test beams.",1404.7046v2 2014-05-07,Thermal effects and switching kinetics in silver/manganite memristive systems: Probing oxygen vacancies diffusion,"We investigate the switching kinetics of oxygen vacancies (Ov) diffusion in LPCMO-Ag memristive interfaces by performing experiments on the temperature dependence of the high resistance (HR) state under thermal cycling. Experimental results are well reproduced by numerical simulations based on thermally activated Ov diffusion processes and fundamental assumptions relying on a recent model proposed to explain bipolar resistive switching in manganite- based cells. The confident values obtained for activation energies and diffusion coefficient associated to Ov dynamics, constitute a validation test for both model predictions and Ov diffusion mechanisms in memristive interfaces.",1405.1585v1 2014-06-26,Signal Characteristics of a Resistive-Strip Micromegas Detector with an Integrated Two-Dimensional Readout,"In recent years, micropattern gaseous detectors, which comprise a two-dimensional readout structure within one PCB layer, received significant attention in the development of precision and cost-effective tracking detectors in medium and high energy physics experiments. In this article, we present for the first time a systematic performance study of the signal characteristics of a resistive strip micromegas detector with a two-dimensional readout, based on test-beam and X-ray measurements. In particular, comparisons of the response of the two independent readout-layers regarding their signal shapes and signal reconstruction efficiencies are discussed.",1406.6871v1 2016-06-25,Linear and quadratic in temperature resistivity from holography,"We present a new black hole solution in the asymptotic Lifshitz spacetime with a hyperscaling violating factor. A novel computational method is introduced to compute the DC thermoelectric conductivities analytically. We find that both the linear-T and quadratic-T contributions to the resistivity can be realized, indicating that a more detailed comparison with experimental phenomenology can be performed in this scenario.",1606.07905v3 2017-02-18,Delta-doped Beta- Gallium Oxide Field Effect Transistor,"We report silicon delta doping in Gallium Oxide (\b{eta}-Ga2O3) grown by plasma assisted molecular beam epitaxy using a shutter pulsing technique. We describe growth procedures that can be used to realize high Si incorporation in an oxidizing oxygen plasma environment. Delta doping was used to realize thin (12 nm) low-resistance layers with sheet resistance of 320 Ohm/square (mobility of 83 cm^2/Vs, integrated sheet charge of 2.4x10^14 cm^-2). A single delta-doped sheet of carriers was employed as a channel to realize a field effect transistor with current ID,MAX =292 mA/mm and transconductance gM = 27 mS/mm.",1702.06584v1 2017-11-17,An HLLC Riemann Solver for Resistive Relativistic Magnetohydrodynamics,"We present a new approximate Riemann solver for the augmented system of equations of resistive relativistic magnetohydrodynamics (RRMHD) that belongs to the family of Harten-Lax-van Leer contact wave (HLLC) solvers. In HLLC solvers, the solution is approximated by two constant states flanked by two shocks separated by a contact wave. The accuracy of the new approximate solver is calibrated through one- and two-dimensional test problems.",1711.06691v2 2018-02-01,MHD simulations of resistive viscous accretion disk around millisecond pulsar,"We perform MHD simulations of a thin resistive and viscous accretion disk around a neutron star with the surface dipolar magnetic field of 10$^8$ Gauss. The system evolution is followed during the interval of 500 millisecond pulsar rotations. Matter is accreted through a stable accretion column from the disk onto the star. We also show propagation of the stellar wind through the corona. Analysis of the mass accretion flux and torques on the star shows that the disk reaches the quasi-stationary state.",1802.00261v1 2014-08-01,Nonmetallic Low-Temperature Normal State of K0.70Fe1.46Se1.85Te0.15,"The normal-state in-plane resistivity below the zero-field superconducting transition temperature $T_c$ and the upper critical field Hc2 were measured by suppressing superconductivity in pulsed magnetic fields for K0.70Fe1.46Se1.85Te0.15. The normal-state resistivity $\rho_{ab}$ is found to increase logarithmically with decrasing temperature as $\frac{T}{T_c}\rightarrow 0$. Similar to granular metals, our results suggest that a superconductor - insulator transition below zero-field T$_{c}$ may be induced in high magnetic fields. This is related to the intrinsic real-space phase-separated states common to all inhomogeneous superconductors.",1408.0271v1 2020-02-22,Accelerating longitudinal expansion of resistive relativistic-magneto-hydrodynamics in heavy ion collisions,"We study the evolution of the longitudinal expansion of an ideal fluid with finite electrical conductivity, which is subject to the EM fields. In the framework of resistive relativistic-magneto-hydrodynamic, we find an exact analytical solution for the EM fields and for the acceleration of the fluid.",2002.09752v1 2012-01-03,Sub-Rayleigh lithography using high flux loss-resistant entangled states of light,"Quantum lithography achieves phase super-resolution using fragile, experimentally challenging entangled states of light. We propose a scalable scheme for creating features narrower than classically achievable, with reduced use of quantum resources and consequently enhanced resistance to loss. The scheme is an implementation of interferometric lithography using a mixture of an SPDC entangled state with intense classical coherent light. We measure coincidences of up to four photons mimicking multiphoton absorption. The results show a narrowing of the interference fringes of up to 30% with respect to the best analogous classical scheme using only 10% of the non-classical light required for creating NOON states.",1201.0637v1 2017-08-02,Graphene membrane as a pressure gauge,"Straining graphene results in the appearance of a pseudo-magnetic field which alters its local electronic properties. Applying a pressure difference between the two sides of the membrane causes it to bend/bulge resulting in a resistance change. We find that the resistance changes linearly with pressure for bubbles of small radius while the response becomes non-linear for bubbles that stretch almost to the edges of the sample. This is explained as due to the strong interference of propagating electronic modes inside the bubble. Our calculations show that high gauge factors can be obtained in this way which makes graphene a good candidate for pressure sensing.",1708.00678v1 2019-12-18,Large responsivity of graphene radiation detectors with thermoelectric readout,"Simple estimations show that the thermoelectric readout in graphene radiation detectors can be extremely effective even for graphene with modest charge-carrier mobility ~1000 cm^2/(Vs). The detector responsivity depends mostly on the residual charge-carrier density and split-gate spacing and can reach competitive values of ~10^3 - 10^4 V/W at room temperature. The optimum characteristics depend on a trade-off between the responsivity and the total device resistance. Finding out the key parameters and their roles allows for simple detectors and their arrays, with high responsivity and sufficiently low resistance matching that of the radiation-receiving antenna structures.",1912.08489v1 2012-03-01,Magnetic and transport properties of iron-platinum arsenide Ca10(Pt4-δAs8)(Fe2-xPtxAs2)5 single crystal,"We report superconducting properties of single crystalline Ca10(Pt4-{\delta}As8)(Fe2-xPtxAs2)5 by X-ray diffraction, magnetization, resistivity, and magneto-optical imaging measurements. The magnetization measurements reveal fish-tail hysteresis loop and relatively high critical current density Jc ~ 0.8\times105 A/cm2 at low temperatures. The exponential temperature dependence of Jc, which arises from nonlinear effective flux-creep activation energy, has been observed. Upper critical field determined by resistive transition shows a relatively large anisotropy. The magneto-optical images reveal homogenous current flow within the crystal.",1203.0099v1 2012-03-22,Tungsten silicide films for microwave kinetic inductance detectors,"Microwave Kinetic Inductance Detectors (MKIDs) provide highly multiplexed arrays of detectors that can be configured to operate from the sub-millimeter to the X-ray regime. We have examined two tungsten silicide alloys (W5Si3 and WSi2), which are dense alloys that provide a critical temperature tunable with composition, large kinetic inductance fraction, and high normal-state resistivity. We have fabricated superconducting resonators and provide measurement data on critical temperature, surface resistance, quality factor, noise, and quasiparticles lifetime. Tungsten silicide appears to be promising for microwave kinetic inductance detectors.",1203.5064v2 2016-09-10,Angular resolution of stacked resistive plate chambers,"We present here detailed derivations of mathematical expressions for the accuracy in the arrival direction of particles estimated using a set of stacked resistive plate chambers (RPCs). The expressions are validated against experimental results using data collected from the prototype detectors (without magnet) of the upcoming India-based Neutrino Observatory (INO). We also present a theoretical estimate of angular resolution of such a setup. In principle, these expressions can be used for any other detector with an architecture similar to that of RPCs.",1609.03071v2 2016-09-19,Scaling limits of stochastic processes associated with resistance forms,"We establish that if a sequence of spaces equipped with resistance metrics and measures converge with respect to the Gromov-Hausdorff-vague topology, and a certain non-explosion condition is satisfied, then the associated stochastic processes also converge. This result generalises previous work on trees, fractals, and various models of random graphs. We further conjecture that it will be applicable to the random walk on the incipient infinite cluster of critical bond percolation on the high-dimensional integer lattice.",1609.05666v1 2020-12-24,Backflow in simulated MHD accretion disks,"We perform resistive MHD simulations of accretion disk with alpha-viscosity, accreting onto a rotating star endowed with a magnetic dipole. We find backflow in the presence of strong magnetic field and large resistivity, and probe for the dependence on Prandtl number. We find that in the magnetic case the distance from the star at which backflow begins, the stagnation radius, is different than in the hydrodynamic case, and the backflow shows non-stationary behavior. We compare the results with hydrodynamics simulations.",2012.13194v1 2021-10-05,Density-Driven Resistance Response in $MnS_{2}$: Theory,"A colossal insulator-to-metal transition in high-spin pyrite phase of $MnS_{2}$ has been experimentally observed \cite{colomns2}. There are two possibilities behind this colossal insulator-to-metal transition: (1) migration of $Mn$ electrons to unoccupied $S^{2-}_{2}$ antibonding states under pressure which leads to conducting ligand states and hence metallic transition, and (2) possibility of band crossing transition. We have analyzed this experimental obervation theoretically using a toy statistical model and found that the transition is due to the migration of electrons from the transition metal ions to the ligand sites (i.e. the possibility (1)). The calculated resistivity compares well with the experimental data within the fitting parameters of the model.",2110.01902v1 2022-07-25,Superconductor--Insulator Transition in a non-Fermi Liquid,"We present a model of a strongly correlated system with a non-Fermi liquid high temperature phase. Its ground state undergoes an insulator to superconductor quantum phase transition (QPT) as a function of a pairing interaction strength. Both the insulator and the superconductor are originating from the same interaction mechanism. The resistivity in the insulating phase exhibits the activation behavior with the activation energy, which goes to zero at the QPT. This leads to a wide quantum critical regime with an algebraic temperature dependence of the resistivity. Upon raising the temperature in the superconducting phase, the model exhibits a finite temperature phase transition to a Bose metal phase, which separates the superconductor from the non-Fermi liquid metal.",2207.12307v1 2024-01-19,Asymptotic behavior of solution of the non-resistive 2D MHD equations on the half space,"In this paper, we obtain the global well-posedness and the asymptotic behavior of solution of non-resistive 2D MHD problem on the half space. We overcome the difficulty of zero spectrum gap by building the relationship between half space and the whole space, and get the resolvent estimate for the weak diffusion system. We use the two-tier energy method that couples the boundedness of high-order $(H^3)$ energy to the decay of low-order energy, the latter of which is necessary to control the growth of the highest energy.",2401.10456v1 2005-03-22,Theoretical current-voltage characteristics of ferroelectric tunnel junctions,"We present the concept of ferroelectric tunnel junctions (FTJs). These junctions consist of two metal electrodes separated by a nanometer-thick ferroelectric barrier. The current-voltage characteristics of FTJs are analyzed under the assumption that the direct electron tunneling represents the dominant conduction mechanism. First, the influence of converse piezoelectric effect inherent in ferroelectric materials on the tunnel current is described. The calculations show that the lattice strains of piezoelectric origin modify the current-voltage relationship owing to strain-induced changes of the barrier thickness, electron effective mass, and position of the conduction-band edge. Remarkably, the conductance minimum becomes shifted from zero voltage due to the piezoelectric effect, and a strain-related resistive switching takes place after the polarization reversal in a ferroelectric barrier. Second, we analyze the influence of the internal electric field arising due to imperfect screening of polarization charges by electrons in metal electrodes. It is shown that, for asymmetric FTJs, this depolarizing-field effect also leads to a considerable change of the barrier resistance after the polarization reversal. However, the symmetry of the resulting current-voltage loop is different from that characteristic of the strain-related resistive switching. The crossover from one to another type of the hysteretic curve, which accompanies the increase of FTJ asymmetry, is described taking into account both the strain and depolarizing-field effects. It is noted that asymmetric FTJs with dissimilar top and bottom electrodes are preferable for the non-volatile memory applications because of a larger resistance on/off ratio.",0503546v1 2013-04-09,Active control of magnetoresistance of organic spin valves using ferroelectricity,"Organic spintronic devices have been appealing because of the long spin life time of the charge carriers in the organic materials and their low cost, flexibility and chemical diversity. In previous studies, the control of resistance of organic spin valves is generally achieved by the alignment of the magnetization directions of the two ferromagnetic electrodes, generating magnetoresistance.1 Here we employ a new knob to tune the resistance of organic spin valves by adding a thin ferroelectric interfacial layer between the ferromagnetic electrode and the organic spacer. We show that the resistance can be controlled by not only the spin alignment of the two ferromagnetic electrodes, but also by the electric polarization of the interfacial ferroelectric layer: the MR of the spin valve depends strongly on the history of the bias voltage which is correlated with the polarization of the ferroelectric layer; the MR even changes sign when the electric polarization of the ferroelectric layer is reversed. This new tunability can be understood in terms of the change of relative energy level alignment between ferromagnetic electrode and the organic spacer caused by the electric dipole moment of the ferroelectric layer. These findings enable active control of resistance using both electric and magnetic fields, opening up possibility for multi-state organic spin valves and shed light on the mechanism of the spin transport in organic spin valves.",1304.2446v2 2017-12-22,The Role of Oxygen in Ionic Liquid Gating on 2D Cr2Ge2Te6: a Non-Oxide Material,"Ionic liquid gating can markedly modulate the materials' carrier density so as to induce metallization, superconductivity, and quantum phase transitions. One of the main issues is whether the mechanism of ionic liquid gating is an electrostatic field effect or an electrochemical effect, especially for oxide materials. Recent observation of the suppression of the ionic liquid gate-induced metallization in the presence of oxygen for oxide materials suggests the electrochemical effect. However, in more general scenarios, the role of oxygen in ionic liquid gating effect is still unclear. Here, we perform the ionic liquid gating experiments on a non-oxide material: two-dimensional ferromagnetic Cr2Ge2Te6. Our results demonstrate that despite the large increase of the gate leakage current in the presence of oxygen, the oxygen does not affect the ionic liquid gating effect (< 5 % difference), which suggests the electrostatic field effect as the mechanism on non-oxide materials. Moreover, our results show that the ionic liquid gating is more effective on the modulation of the channel resistances compared to the back gating across the 300 nm thick SiO2.",1712.08281v1 2022-11-30,Anomalous magneto-thermoelectric behavior in massive Dirac materials,"Extensive studies of electron transport in Dirac materials have shown positive magneto-resistance (MR) and positive magneto-thermopower (MTP) in a magnetic field perpendicular to the excitation current or thermal gradient. In contrast, measurements of electron transport often show a negative longitudinal MR and negative MTP for a magnetic field oriented along the excitation current or thermal gradient; this is attributed to the chiral anomaly in Dirac materials. Here, we report a very different magneto-thermoelectric transport behavior in the massive Dirac material ZrTe5. Although thin flakes show a commonly observed positive MR in a perpendicular magnetic field, distinct from other Dirac materials, we observe a sharp negative MTP. In a parallel magnetic field, we still observe a negative longitudinal MR, however, a remarkable positive MTP is observed for the fields parallel to the thermal gradients. Our theoretical calculations suggest that this anomalous magneto-thermoelectric behavior can be attributed to the screened Coulomb scattering. This work demonstrates the significance of impurity scattering in the electron transport of topological materials and provides deep insight into the novel magneto-transport phenomena in Dirac materials.",2211.17027v1 2022-12-01,Process parameter sensitivity of the energy absorbing properties of additively manufactured metallic cellular materials,"Additive Manufacturing (AM) has enabled the fabrication of metallic cellular materials that are of interest in the design of lightweight impact resistant structures. However, there is a need to understand the interactions between: (i) the material architecture, (ii) the AM process parameters, and (iii) the as-built geometry, microstructure and energy absorbing properties. In this work, we investigate the quasi-static and dynamic behaviour of cellular materials manufactured from 316L stainless steel using laser powder bed fusion (LPBF). Four cellular architectures are considered (octet lattice, lattice-walled square honeycomb, origami and square honeycomb), as well as three sets of AM process parameters, characterised by laser powers of 50, 125 and 200 W. The exposure time is adjusted to deliver the same total heat input. The 125 W case leads to material with the highest strength and ductility. The cellular materials with this process variant match their nominal densities most closely, and have the highest strength and energy absorption. Either reducing (50 W) or increasing (200 W) the power leads to a significant increase in porosity, reducing strength and energy absorption. However, we find that changes due to process-induced porosity have a smaller influence than those resulting from the choice of cellular architecture.",2212.00438v1 2023-09-11,Button Shear Testing for Adhesion Measurements of 2D Materials,"Two-dimensional (2D) materials are considered for numerous applications in microelectronics, although several challenges remain when integrating them into functional devices. Weak adhesion is one of them, caused by their chemical inertness. Quantifying the adhesion of 2D materials on three-dimensional surfaces is, therefore, an essential step toward reliable 2D device integration. To this end, button shear testing is proposed and demonstrated as a method for evaluating the adhesion of 2D materials with the examples of graphene and hexagonal boron nitride (hBN), molybdenum disulfide, and tungsten diselenide on silicon dioxide (SiO${_2}$) and silicon nitride substrates. We propose a fabrication process flow for polymer buttons on the 2D materials and establish suitable button dimensions and testing shear speeds. We show with our quantitative data that low substrate roughness and oxygen plasma treatments on the substrates before 2D material transfer result in higher shear strengths. Thermal annealing increases the adhesion of hBN on SiO${_2}$ and correlates with the thermal interface resistance between these materials. This establishes button shear testing as a reliable and repeatable method for quantifying adhesion of 2D materials.",2309.05852v3 1997-05-09,Small-q electron-phonon scattering and linear dc resistivity in high-T_c oxides,"We examine the effect on the DC resistivity of small-q electron-phonon scattering, in a system with the electronic topology of the high-T_c oxides. Despite the fact that the scattering is dominantly forward, its contribution to the transport can be significant due to ``ondulations'' of the bands in the flat region and to the umpklapp process. When the extended van-Hove singularities are sufficiently close to $E_F$ the acoustic branch of the phonons contribute significantly to the transport. In that case one can obtain linear $T$ dependent resistivity down to temperatures as low as 10 K, even if electrons are scattered also by optical phonons of about 500 K as reported by Raman measurements.",9705085v1 1999-05-14,Universal scaling of Hall resistivity in clean and moderately clean limits for Hg- and Tl-based superconductors,"The mixed-state Hall resistivity and the longitudinal resistivity in HgBa_{2}CaCu_{2}O_{6}, HgBa_{2}Ca_{2}Cu_{3}O_{8}, and Tl_{2}Ba_{2}CaCu_{2}O_{8} thin films have been investigated as functions of the magnetic field up to 18 T. We observe the universal scaling behavior between \rho_{xy} and \rho_{xx} in the regions of the clean and the moderately clean limit. The scaling exponent \beta is 1.9 in the clean limit at high field and low temperature whereas \beta is 1.0 in the moderately clean limit at low field and high temperature, consistent with a theory based on the midgap states in the vortex cores. This finding implies that the Hall conductivity is also universal in Hg- and Tl-based superconductors.",9905201v1 1999-10-04,Normal State Resistivity of Underdoped YBa2Cu3Ox Thin Films and La2-xSrxCuO4 Ultra-Thin Films under Epitaxial Strain,"The normal state resistivity of high temperature superconductors can be probed in the region below Tc by suppressing the superconducting state in high magnetic fields. Here we present the normal state properties of YBa2Cu3Ox thin films in the underdoped regime and the normal state resistance of La2-xSrxCuO4 thin films under epitaxial strain, measured below Tc by applying pulsed fields up to 60 T. A universal rho(T) behaviour is reported. We interpret these data in terms of the recently proposed 1D quantum transport model with the 1D paths corresponding to the charge stripes.",9910033v1 2001-03-04,Effect of the In-Plane Magnetic Field on Conduction of the Si-inversion Layer: Magnetic Field Driven Disorder,"We compare the effects of temperature, disorder and parallel magnetic field on the metallic-like temperature dependence of the resistivity. We found a similarity between the effects of disorder and parallel field: the parallel field weakens the metallic-like conduction in high mobility samples and make it similar to that for low-mobility samples. We found a smooth continuous effect of the in-plane field on conduction, without any threshold. While conduction remains non-activated, the parallel magnetic field restores the same resistivity value as the high temperature does. This matching sets substantial constraints on the choice of the theoretical models developed to explain the mechanism of the metallic conduction and parallel field magnetoresistance in 2D carrier systems. We demonstrate that the data for magneto- and temperature dependence of the resistivity of Si-MOS samples in parallel field may be well described by a simple model of the magnetic field dependent disorder.",0103087v2 2001-11-20,High-pressure study on the superconducting pyrochlore oxide Cd2Re2O7,"Superconducting and structural phase transitions in a pyrochlore oxide Cd2Re2O7 are studied under high pressure by x-ray diffraction and electrical resistivity measurements. A rich P-T phase diagram is obtained, which contains at least two phases with the ideal and slightly distorted pyrochlore structures. It is found that the transition between them is suppressed with increasing pressure and finally disappears at a critical pressure Pc = 3.5 GPa. Remarkable enhancements in the residual resistivity as well as the coefficient A of the AT 2 term in the resistivity are found around the critical pressure. Superconductivity is detected only for the phase with the structural distortion. It is suggested that the charge fluctuations of Re ions play a crucial role in determining the electronic properties of Cd2Re2O7.",0111388v2 2002-10-02,Two-band effects in transport properties of MgB2,"We present resistivity and thermal conductivity measurements on bulk samples, prepared either by a standard method or by a one-step technique. The latter samples, due to their high density and purity, show residual resistivity values as low as 0.5 mW cm and thermal conductivity values as high as 215 W/mK, higher than the single crystal ones. Thermal and electrical data of all the samples are analysed in the framework of the Bloch-Gruneisen equation giving reliable parameter values. In particular the temperature resitivity coefficient, obtained both from resistivity and thermal conductivity, in the dirty sample comes out ten time larger than in the clean ones. This result supports the hypothesis of ref. [1] that p and s bands conduct in parallel, prevailing p conduction in clean samples and s conduction in dirty samples .",0210047v2 2003-07-31,Radiation-intensity and temperature dependence of microwave-induced magnetoresistance oscillations in high-mobility two-dimensional electron systems,"We present a detailed theoretical investigation on the radiation induced giant magnetoresistance oscillations recently discovered in high-mobility two-dimensional electron gas. Electron interactions with impurities, transverse and longitudinal acoustic phonons in GaAs-based heterosystems are considered simultaneously. Multiphoton-assisted impurity scatterings are shown to be the primary origin of the resistance oscillation. Based on the balance-equation theory developed for magnetotransport in Faraday geometry, we are able not only to reproduce the observed period, phase and the negative resistivity of the main oscillations, but also to predict the secondary peak/valley structures relating to two-photon and three-photon processes. The dependence of the magnetoresistance oscillation on microwave intensity, the role of dc bias current and the effect of elevated electron temperature are discussed. Furthermore, we propose that the temperature-dependence of the resistance oscillation stems from the growth of the Landau level broadening due to the enhancement of acoustic phonon scattering with increasing lattice temperature. The calculated temperature-variation of the oscillation agrees well with experimental observations.",0307757v1 2003-09-29,Andreev reflection and enhanced subgap conductance in NbN/Au/InGaAs-InP junctions,"We report on the fabrication of highly transparent superconductor/normal metal/two-dimensional electron gas junctions formed by a superconducting NbN electrode, a thin (10nm) Au interlayer, and a two-dimensional electron gas in a InGaAs/InP heterostructure. High junction transparency has been achieved by exploiting of a newly developed process of Au/NbN evaporation and rapid annealing at 400C. This allowed us to observe for the first time a decrease in the differential resistance with pronounced double-dip structure within the superconducting energy gap in superconductor-2DEG proximity systems. The effect of a magnetic field perpendicular to the plane of the 2DEG on the differential resistance of the interface was studied. It has been found that the reduced subgap resistance remains in high magnetic fields. Zero-field data are analyzed within the previously established quasiclassical model for the proximity effect.",0309682v2 2004-01-07,Large positive magneto-resistance in high mobility 2D electron gas : interplay of short and long range disorder,"We have observed a large positive quasi-classical magneto-resistance (MR) in a high mobility 2D electron gas in AlGaAs/GaAs heterostructure. The magneto-resistance is non-saturating and increases with magnetic field as $\rho_{xx}\sim B^{\alpha} (\alpha=0.9-1.2)$. In antidot lattices a non-monotonic MR is observed. We show that in both cases this MR can be qualitatively described in terms of the theory recently advanced by Polyakov et al (PRB, 64, 205306 (2001)). Their prediction is that such behavior as we observe may be the consequence of a concurrent existence of short and long range scattering potentials.",0401085v2 2004-03-01,Electronic Phase Diagram of High-T_c Cuprate Superconductors from a Mapping of the In-Plane Resistivity Curvature,"We propose that Resistivity Curvature Mapping (RCM) based on the in-plane resistivity data is a useful way to objectively draw an electronic phase diagrams of high-T_c cuprates, where various crossovers are important. In particular, the pseudogap crossover line can be conveniently determined by RCM. We show experimental phase diagrams obtained by RCM for Bi_{2}Sr_{2-z}La_{z}CuO_{6+\delta}, La_{2-x}Sr_{x}CuO_{4}, and YBa_{2}Cu_{3}O_{y}, and demonstrate the universal nature of the pseudogap crossover. Intriguingly, the electronic crossover near optimum doping depicted by RCM appears to occur rather abruptly, suggesting that the quantum critical regime, if exists, must be very narrow.",0403032v2 2004-12-15,The resistive transition and Meissner effect in carbon nanotubes: Evidence for quasi-one-dimensional superconductivity above room temperature,"It is well known that copper-based perovskite oxides rightly enjoy consensus as high-temperature superconductors on the basis of two signatures: the resistive transition and the Meissner effect. We show that the resistive transitions in carbon nanotubes agree quantitatively with the Langer-Ambegaokar-McCumber-Halperin (LAMH) theory for quasi-1D superconductors although the superconducting transition temperatures can vary from 0.4 K to 750 K for different samples. We have also identified the Meissner effect in the field parallel to the tube axis up to room temperature for aligned and physically separated multi-walled nanotubes (MWNTs). The magnitude of the Meissner effect is in quantitative agreement with the predicted penetration depth from the measured carrier density. Furthermore, the bundling of individual MWNTs into closely packed bundles leads to a large enhancement in the diamagnetic susceptibility, which is the hallmark of the Josephson coupling among the tubes in bundles. These results consistently indicate quasi-1D high-temperature superconductivity in carbon nanotubes.",0412382v2 2005-02-09,Low-temperature nodal-quasiparticle transport in lightly doped YBa_{2}Cu_{3}O_{y} near the edge of the superconducting doping regime,"In-plane transport properties of nonsuperconducting YBa_{2}Cu_{3}O_{y} (y = 6.35) are measured using high-quality untwinned single crystals. We find that both the a- and b-axis resistivities show log(1/T) divergence down to 80 mK, and accordingly the thermal conductivity data indicate that the nodal quasiparticles are progressively localized with lowering temperature. Hence, both the charge and heat transport data do not support the existence of a ""thermal metal"" in nonsuperconducting YBa_{2}Cu_{3}O_{y}, as opposed to a recent report by Sutherland {\it et al.} [Phys. Rev. Lett. {\bf 94}, 147004 (2005)]. Besides, the present data demonstrate that the peculiar log(1/T) resistivity divergence of cuprate is {\it not} a property associated with high-magnetic fields.",0502223v2 2006-04-19,Transport Properties of Granular High-TC Superconductors,"We report on the application of the Resistively Shunted Junction (RSJ) model to granular high-TC superconductors. Some derived predictions of the RSJ model are applied to a set of superconducting granular samples which can be considered as a network of Josephson junctions. The investigated samples belong to both hole-doped Y1-xPrxBa2Cu3O7-d (x = 0.0, 0.35, and 0.45) and the electron-doped Sm2-xCexCuO4-d (x = 0.18) systems which display the so-called double resistive superconducting transition. We have performed several transport measurements in these compounds including temperature and magnetic field dependence of the electrical resistance, R(T,H), and I-V characteristics. Several aspects of the I-V characteristics were quantitatively well described by the RSJ model. The combined results strongly suggest that dissipation in granular superconducting samples is a natural consequence of the normal current flowing in parallel with the supercurrent current.",0604460v1 2006-10-05,Unconventional resistivity at the border of metallic antiferromagnetism in NiS2,"We report low-temperature and high-pressure measurements of the electrical resistivity \rho(T) of the antiferromagnetic compound NiS_2 in its high-pressure metallic state. The form of \rho(T) suggests that metallic antiferromagnetism in NiS_2 is quenched at a critical pressure p_c=76+-5 kbar. Near p_c the temperature variation of \rho(T) is similar to that observed in NiS_{2-x}Se_x near the critical composition x=1 where the Neel temperature vanishes at ambient pressure. In both cases \rho(T) varies approximately as T^{1.5} over a wide range below 100 K. However, on closer analysis the resistivity exponent in NiS_2 exhibits an undulating variation with temperature not seen in NiSSe (x=1). This difference in behaviour may be due to the effects of spin-fluctuation scattering of charge carriers on cold and hot spots of the Fermi surface in the presence of quenched disorder, which is higher in NiSSe than in stoichiometric NiS_2.",0610166v1 2009-05-29,Ferromagnetic quantum phase transition in Sr$_{1-x}$Ca$_x$RuO$_3$ thin films,"The ferromagnetic quantum phase transition in the perovskite ruthenate Sr$_{1-x}$Ca$_x$RuO$_3$ is studied by low-temperature magnetization and electrical resistivity measurements on thin films. The films were grown epitaxially on SrTiO$_3$ substrates using metalorganic aerosol deposition and characterized by X-ray diffraction and room temperature scanning tunneling microscopy. High residual resistivity ratios of 29 and 16 for $x=0$ and $x=1$, respectively, prove the high quality of the investigated samples. We observe a continuous suppression of the ferromagnetic Curie temperature from $T_C=160$ K at $x=0$ towards $T_C\to 0$ at $x_c\approx 0.8$. The analysis of the electrical resistivity between 2 and 10 K reveals $T^2$ and $T^{3/2}$ behavior at $x\leq 0.6$ and $x\geq 0.7$, respectively. For undoped CaRuO$_3$, the measurement has been extended down to 60 mK, revealing a crossover to $T^2$ behavior around 2 K, which suggests a Fermi-liquid ground state in this system.",0905.4885v1 2009-08-10,Temperature Dependence of Magnetophonon Resistance Oscillations in GaAs/AlAs Heterostructures at High Filling Factors,"The temperature dependence of phonon-induced resistance oscillations has been investigated in two-dimensional electron system with moderate mobility at large filling factors at temperature range T = 7.4 - 25.4 K. The amplitude of phonon-induced oscillations has been found to be governed by quantum relaxation time which is determined by electron-electron interaction effects. This is in agreement with results recently obtained in ultra-high mobility two-dimensional electron system with low electron density [A. T. Hatke et al., Phys. Rev. Lett. 102, 086808 (2009)]. The shift of the main maximum of the magnetophonon resistance oscillations to higher magnetic fields with increasing temperature is observed.",0908.1293v2 2009-10-09,Electromagnetic response of LaO_0.94F_0.06FeAs: AC susceptibility and microwave surface resistance,"We discuss on the electromagnetic response of a polycrystalline sample of LaO_0.94F_0.06FeAs exposed to DC magnetic fields up to 10 kOe. The low- and high-frequency responses have been investigated by measuring the AC susceptibility at 100 kHz and the microwave surface resistance at 9.6 GHz. At low as well as high DC magnetic fields, the susceptibility strongly depends on the amplitude of the AC driving field, highlighting enhanced nonlinear effects. The field dependence of the AC susceptibility exhibits a magnetic hysteresis that can be justified considering the intragrain-field-penetration effects on the intergrain critical current density. The microwave surface resistance exhibits a clockwise magnetic hysteresis, which cannot be justified in the framework of the critical-state models of the Abrikosov-fluxon lattice; it may have the same origin as that detected in the susceptibility.",0910.1805v1 2010-08-04,High-Pressure Electrical Resistivity Measurements of EuFe2As2 Single Crystals,"High-pressure electrical resistivity measurements up to 3.0GPa have been performed on EuFe2As2 single crystals with residual resistivity ratios RRR=7 and 15. At ambient pressure, a magnetic / structural transition related to FeAs-layers is observed at T0 =190K and 194K for samples with RRR=7 and 15, respectively. Application of hydrostatic pressure suppresses T0, and then induces similar superconducting behavior in the samples with different RRR values. However, the critical pressure 2.7GPa, where T0=0, for the samples with RRR=15 is slightly but distinctly larger than 2.5GPa for the samples with RRR=7.",1008.0684v1 2010-12-26,Superconductivity at 32 K in single crystal Rb$_{0.78}$Fe$_2$Se$_{1.78}$},"We successfully grew the high-quality single crystal of Rb$_{0.78}$Fe$_2$Se$_{1.78}$, which shows sharp superconducting transition in magnetic susceptibility and electrical resistivity. Resistivity measurements show the onset superconducting transition ($T_{\rm c}$) at 32.1 K and zero resistivity at 30 K. From the low-temperature iso-magnetic-field magnetoresistance, large upper critical field $H_{\rm c2}$(0) has been estimated as high as 180 T for in-plane field and 59 T for out-of-plane field. The anisotropy $H^{ab}_{\rm c2}$(0)/$H^{c}_{\rm c2}$(0) is around 3.0, right lying between those observed in K$_x$Fe$_2$Se$_2$ and Cs$_x$Fe$_2$Se$_2$.",1012.5525v1 2012-07-23,Quantum oscillations and high carrier mobility in the delafossite PdCoO$_2$,"We present de Haas-van Alphen and resistivity data on single crystals of the delafossite PdCoO2. At 295 K we measure an in-plane resistivity of 2.6 \mu{\Omega}-cm, making PdCoO2 the most conductive oxide known. The low-temperature in-plane resistivity has an activated rather than the usual T^5 temperature dependence, suggesting a gapping of effective scattering that is consistent with phonon drag. Below 10 K, the transport mean free path is 20 \mum, approximately 10^5 lattice spacings and an astoundingly high value for flux-grown crystals. We discuss the origin of these properties in light of our data.",1207.5402v1 2012-10-02,Magnetotransport in graphene on silicon side of SiC,"We have studied the transport properties of graphene grown on silicon side of SiC. Samples under study have been prepared by two different growth methods in two different laboratories. Magnetoresistance and Hall resistance have been measured at temperatures between 4 and 100 K in resistive magnet in magnetic fields up to 22 T. In spite of differences in sample preparation, the field dependence of resistances measured on both sets of samples exhibits two periods of magneto-oscillations indicating two different parallel conducting channels with different concentrations of carriers. The semi-quantitative agreement with the model calculation allows for conclusion that channels are formed by high-density and low-density Dirac carriers. The coexistence of two different groups of carriers on the silicon side of SiC was not reported before.",1210.0744v2 2013-01-02,Plasmoid Instability in High-Lundquist-Number Magnetic Reconnection,"Our understanding of magnetic reconnection in resistive magnetohydrodynamics has gone through a fundamental change in recent years. The conventional wisdom is that magnetic reconnection mediated by resistivity is slow in laminar high Lundquist ($S$) plasmas, constrained by the scaling of the reconnection rate predicted by Sweet-Parker theory. However, recent studies have shown that when $S$ exceeds a critical value $\sim10^{4}$, the Sweet-Parker current sheet is unstable to a super-Alfv\'enic plasmoid instability, with a linear growth rate that scales as $S^{1/4}$. In the fully developed statistical steady state of two-dimensional resistive magnetohydrodynamic simulations, the normalized average reconnection rate is approximately 0.01, nearly independent of $S$, and the distribution function $f(\psi)$ of plasmoid magnetic flux $\psi$ follows a power law $f(\psi)\sim\psi^{-1}$. When Hall effects are included, the plasmoid instability may trigger onset of Hall reconnection even when the conventional criterion for onset is not satisfied. The rich variety of possible reconnection dynamics is organized in the framework of a phase diagram.",1301.0331v2 2013-02-09,mrPUF: A Memristive Device based Physical Unclonable Function,"Physical unclonable functions (PUFs) exploit the intrinsic complexity and irreproducibility of physical systems to generate secret information. PUFs have the potential to provide fundamentally higher security than traditional cryptographic methods by preventing the cloning of identities and the extraction of secret keys. One unique and exciting opportunity is that of using the super-high information content (SHIC) capability of nanocrossbar architecture as well as the high resistance programming variation of resistive memories to develop a highly secure on-chip PUFs for extremely resource constrained devices characterized by limited power and area budgets such as passive Radio Frequency Identification (RFID) devices. We show how to implement PUF based on nano-scale memristive (resistive memory) devices (mrPUF). Our proposed architecture significantly increased the number of possible challenge-response pairs (CRPs), while also consuming relatively lesser power (around 70 uW). The presented approach can be used in other silicon-based PUFs as well.",1302.2191v1 2013-04-24,A highly resistive layer within the crust of X-ray pulsars limits their spin periods,"The lack of X-ray pulsars with spin periods > 12 s raises the question of where the population of evolved high magnetic field neutron stars has gone. Unlike canonical radio pulsars, X-ray pulsars are not subject to physical limits to the emission mechanism nor observational biases against the detection of sources with longer periods. Here we show that a highly resistive layer in the innermost part of the crust of neutron stars naturally limits the spin period to a maximum value of about 10-20 s. This highly resistive layer is expected if the inner crust is amorphous and heterogeneous in nuclear charge, possibly due to the existence of a nuclear pasta phase. Our findings suggest that the maximum period of isolated X-ray pulsars can be the first observational evidence of an amorphous inner crust, which properties can be further constrained by future X-ray timing missions combined with more detailed models.",1304.6546v2 2014-05-05,Hall field-induced resistance oscillations in Ge/SiGe quantum wells,"We report on a magnetotransport study in a high-mobility 2D hole gas hosted in a pure Ge/SiGe quantum well subject to dc electric fields and high frequency microwave radiation. We find that under applied dc bias the differential resistivity exhibits a pronounced maximum at a magnetic field which increases linearly with the applied current. We associate this maximum with the fundamental peak of Hall field-induced resistance oscillations (HIRO) which are known to occur in 2D electron gases in GaAs/AlGaAs systems. After taking into account the Dingle factor correction, we find that the position of the HIRO peak is well described by the hole effective mass $m^\star \approx 0.09\,m_0$, obtained from microwave photoresistance in the same sample.",1405.1093v1 2014-07-28,An apparent metal insulator transition in high mobility 2D InAs heterostructures,"We report on the first experimental observation of an apparent metal insulator transition in a 2D electron gas confined in an InAs quantum well. At high densities we find that the carrier mobility is limited by background charged impurities and the temperature dependence of the resistivity shows a metallic behavior with resistivity increasing with increasing temperature. At low densities we find an insulating behavior below a critical density of $n_{c} = 5 \times 10^{10}$ cm$^{-2}$ with the resistivity decreasing with increasing temperature. We analyze this transition using a percolation model arising from the failure of screening in random background charged impurities. We also examine the percolation transition experimentally by introducing remote ionized impurities at the surface. Using a bias during cool-down, we modify the screening charge at the surface which strongly affects the critical density. Our study shows that transition from a metallic to an insulating phase in our system is due to percolation transition.",1407.7541v3 2014-11-01,Unusual resistance-voltage dependence of nanojunctions during electromigration in ultra-high vacuum,"The electrical resistance R of metallic nanocontacts subjected to controlled cyclic electromigration in ultra-high vacuum has been investigated in-situ as a function of applied voltage V. For sufficiently small contacts, i.e., large resistance, a decrease of R(V) while increasing V is observed. This effect is tentatively attributed to the presence of contacts separated by thin vacuum barriers in parallel to ohmic nanocontacts. Simple model calculations indicate that both thermal activation or tunneling can lead to this unusual behavior. We describe our data by a tunneling model whose key parameter, i.e., the tunneling distance, changes because of thermal expansion due to Joule heating and/or electrostatic strain arising from the applied voltage. Oxygen exposure during electromigration prevents the formation of negative R(V) slopes, and at the same time enhances the probability of uncontrolled melting, while other gases show little effects. In addition, indication for field emission has been observed in some samples",1411.0105v1 2015-01-15,High Pressure Measurements of the Resistivity of $β$-YbAlB$_4$,"The electric resistivity $\rho(T)$ under hydrostatic pressure up to 8 GPa was measured above 2 K using a high-quality single crystal of the Yb-based heavy fermion system $\beta$-YbAlB$_4$. We found pressure-induced magnetic ordering above the critical pressure $P_{\rm c} \approx $ 2.4 GPa. This phase transition temperature $T_M$ is enhanced with pressure and reaches 30 K at a pressure of 8 GPa, which is the highest transition temperature for the Yb-based heavy fermion compounds. In contrast, the resistivity is insensitive to pressure below $P_c$ and exhibits the $T$-linear behavior in the temperature range between 2 and 20 K. Our results indicate that quantum criticality for $\beta$-YbAlB$_4$ is also located near $P_{\rm c}$ in addition to the ambient pressure.",1501.03852v1 2015-12-17,Alfvén Wave Heating of the Solar Chromosphere: 1.5D models,"Physical processes which may lead to solar chromospheric heating are analyzed using high-resolution 1.5D non-ideal MHD modelling. We demonstrate that it is possible to heat the chromospheric plasma by direct resistive dissipation of high-frequency Alfv\'en waves through Pedersen resistivity. However this is unlikely to be sufficient to balance radiative and conductive losses unless unrealistic field strengths or photospheric velocities are used. The precise heating profile is determined by the input driving spectrum since in 1.5D there is no possibility of Alfv\'en wave turbulence. The inclusion of the Hall term does not affect the heating rates. If plasma compressibility is taken into account, shocks are produced through the ponderomotive coupling of Alfv\'en waves to slow modes and shock heating dominates the resistive dissipation. In 1.5D shock coalescence amplifies the effects of shocks and for compressible simulations with realistic driver spectra the heating rate exceeds that required to match radiative and conductive losses. Thus while the heating rates for these 1.5D simulations are an overestimate they do show that ponderomotive coupling of Alfv\'en waves to sound waves is more important in chromospheric heating than Pedersen dissipation through ion-neutral collisions.",1512.05816v1 2016-02-14,Ultra-sensitive nanoscale magnetic field sensors based on resonant spin filtering,"Solid state magnetic field sensors based on magneto-resistance modulation find direct applications in communication devices, specifically in proximity detection, rotational reference detection and current sensing. In this work, we propose sensor structures based on the magneto-resistance physics of resonant spin-filtering and present device designs catered toward exceptional magnetic field sensing capabilities. Using the non-equilibrium Green's function spin transport formalism self consistently coupled to the Poisson's equation, we present highly-tunable pentalayer magnetic tunnel junction structures that are capable of exhibiting an ultra-high peak tunnel magneto resistance $(\approx 2500 \%$). We show how this translates to device designs featuring an ultra-high current sensitivity enhancement of over 300\% in comparison with typical trilayer MTJ sensors, and a wider tunable range of field sensitivity. We also demonstrate that a dynamic variation in sensor functionalities with the structural landscape enables a superior design flexibility over typical trilayer sensors. An optimal design exhibiting close to a 700\% sensitivity increase as a result of angle dependent spin filtering is then presented.This work sets a stage to engineer spintronic building blocks via the design of functional structures tailored to exhibit ultra-sensitive spin filtering.",1602.04438v1 2016-04-10,Terahertz-induced resistance oscillations in high mobility two-dimensional electron systems,"We report on a theoretical work on magnetotransport under terahertz radiation with high mobility two-dimensional electron systems. We focus on the interaction between the obtained radiation-induced magnetoresistance oscillations (RIRO) and the Shubnikov-de Haas (SdHO) oscillations. We study two effects experimentally obtained with this radiation. First, the observed disappearance of the SdHO oscillations simultaneously with the vanishing resistance at the zero resistance states region. And secondly the strong modulation of the SdHO oscillations at sufficient terahertz radiation power. We conclude that both effects share the same physical origin, the interference between the average advanced distance by the scattered electron between irradiated Landau states, (RIRO), and the available initial density of states at a certain magnetic field, (SdHO). Thus, from a physical standpoint, what the terahertz experiments and theoretical simulations reveal is, on the one hand, the oscillating nature of the Landau states subjected to radiation and, on the other hand, how they behave in the presence of scattering.",1604.02721v1 2016-05-12,Improved Contacts to MoS2 Transistors by Ultra-High Vacuum Metal Deposition,"The scaling of transistors to sub-10 nm dimensions is strongly limited by their contact resistance (Rc). Here we present a systematic study of scaling MoS2 devices and contacts with varying electrode metals and controlled deposition conditions, over a wide range of temperatures (80 to 500 K), carrier densities (10^12 to 10^13 1/cm^2), and contact dimensions (20 to 500 nm). We uncover that Au deposited in ultra-high vacuum (~10^-9 Torr) yields three times lower Rc than under normal conditions, reaching 740 Ohm-um and specific contact resistivity 3x10^-7 Ohm.cm2, stable for over four months. Modeling reveals separate Rc contributions from the Schottky barrier and the series access resistance, providing key insights on how to further improve scaling of MoS2 contacts and transistor dimensions. The contact transfer length is ~35 nm at 300 K, which is verified experimentally using devices with 20 nm contacts and 70 nm contact pitch (CP), equivalent to the ""14 nm"" technology node.",1605.03972v2 2016-10-03,A variational approach to resistive relativistic plasmas,"We develop an action principle to construct the field equations for a multi-fluid system containing charge-neutral fluids, plasmas, and dissipation (via resistive interactions), by combining the standard, Maxwell action and minimal coupling of the electromagnetic field with a recently developed action for relativistic dissipative fluids. We use a pull-back formalism from spacetime to abstract matter spaces to build unconstrained variations for both the charge-neutral fluids and currents making up the plasmas. Using basic linear algebra techniques, we show that a general ""relabeling"" invariance exists for the abstract matter spaces. With the field equations in place, a phenomenological model for the resistivity is developed, using as constraints charge conservation and the Second Law of Thermodynamics. A minimal model for a system of electrons, protons, and heat is developed using the Onsager procedure for incorporating dissipation.",1610.00445v1 2017-02-06,Semiempirical Modeling of Reset Transitions in Unipolar Resistive-Switching Based Memristors,"We have measured the transition process from the high to low resistivity states, i.e., the reset process of resistive switching based memristors based on Ni/HfO2/Si-n+ structures, and have also developed an analytical model for their electrical characteristics. When the characteristic curves are plotted in the current-voltage (I-V) domain a high variability is observed. In spite of that, when the same curves are plotted in the charge-flux domain (Q-f), they can be described by a simple model containing only three parameters: the charge (Qrst) and the flux (frst) at the reset point, and an exponent, n, relating the charge and the flux before the reset transition. The three parameters can be easily extracted from the Q-f plots. There is a strong correlation between these three parameters, the origin of which is still under study.",1702.01533v1 2017-02-28,Evidence for conventional superconductivity in Sr0.1Bi2Se3 from high pressure studies,"SrxBi2Se3 is recently reported to be a superconductor derived from topological insulator Bi2Se3. It shows a maximum resistive Tc of 3.25 K at ambient pressure. We report magnetic (upto 1 GPa) and transport properties (upro 8 Gpa) under pressure for single crystalline Sr0.1Bi2Se3 superconductor. Magnetic measurements show that Tc decreases from ~2.6 K (0 GPa) to ~1.9 K (0.81 GPa). Similar behavior is observed in transport properties as well without much change in the metallic characteristics in normal state resistivity. No reentrant superconducting phase (Physical Review B 93, 144514 (2016)) is observed at high pressure. Normal state resistivity near Tc is explained by Fermi liquid model. Above 100 K, a polaronic hopping conduction mechanism with two parallel channels for current flow is indicated. Band structure calculations indicate decreasing density of states at Fermi level with pressure. In consonance with transition temperature suppression in conventional BCS low Tc superconductors, the pressure effect in SrxBi2Se3 is well accounted by pressure induced band broadening.",1702.08829v1 2017-12-21,"DC resistivity of quantum critical, charge density wave states from gauge-gravity duality","In contrast to metals with weak disorder, the resistivity of weakly-pinned charge density waves (CDWs) is not controlled by irrelevant processes relaxing momentum. Instead, the leading contribution is governed by incoherent, diffusive processes which do not drag momentum and can be evaluated in the clean limit. We compute analytically the dc resistivity for a family of holographic charge density wave quantum critical phases and discuss its temperature scaling. Depending on the critical exponents, the ground state can be conducting or insulating. We connect our results to dc electrical transport in underdoped cuprate high $T_c$ superconductors. We conclude by speculating on the possible relevance of unstable, semi-locally critical CDW states to the strange metallic region.",1712.07994v2 2018-09-27,p-GaAs nanowire MESFETs with near-thermal limit gating,"Difficulties in obtaining high-performance p-type transistors and gate insulator charge-trapping effects present two major challenges for III-V complementary metal-oxide semiconductor (CMOS) electronics. We report a p-GaAs nanowire metal-semiconductor field-effect transistor (MESFET) that eliminates the need for a gate insulator by exploiting the Schottky barrier at the metal-GaAs interface. Our device beats the best-performing p-GaSb nanowire metal-oxide-semiconductor field effect transistor (MOSFET), giving a typical sub-threshold swing of 62 mV/dec, within 4% of the thermal limit, on-off ratio $\sim 10^{5}$, on-resistance ~700 k$\Omega$, contact resistance ~30 k$\Omega$, peak transconductance 1.2 $\mu$S/$\mu$m and high-fidelity ac operation at frequencies up to 10 kHz. The device consists of a GaAs nanowire with an undoped core and heavily Be-doped shell. We carefully etch back the nanowire at the gate locations to obtain Schottky-barrier insulated gates whilst leaving the doped shell intact at the contacts to obtain low contact resistance. Our device opens a path to all-GaAs nanowire MESFET complementary circuits with simplified fabrication and improved performance.",1809.10479v1 2018-10-07,High-resolution disruption halo current measurements using Langmuir probes in Alcator C-Mod,"Halo currents generated during disruptions on Alcator C-Mod have been measured with Langmuir ""rail"" probes. These rail probes are embedded in a lower outboard divertor module in a closely-spaced vertical (poloidal) array. The dense array provides detailed resolution of the spatial dependence (~1 cm spacing) of the halo current distribution in the plasma scrape-off region with high time resolution (400 kHz digitization rate). As the plasma limits on the outboard divertor plate, the contact point is clearly discernible in the halo current data (as an inversion of current) and moves vertically down the divertor plate on many disruptions. These data are consistent with filament reconstructions of the plasma boundary, from which the edge safety factor of the disrupting plasma can be calculated. Additionally, the halo current ""footprint"" on the divertor plate is obtained and related to the halo flux width. The voltage driving halo current and the effective resistance of the plasma region through which the halo current flows to reach the probes are also investigated. Estimations of the sheath resistance and halo region resistivity and temperature are given. This information could prove useful for modeling halo current dynamics.",1810.03207v1 2020-04-27,The Resistivity of High-Tc Cuprates,"We show that the resistivity in each phase of the High-Tc cuprates is a special case of a general expression derived from the Kubo formula. We obtain, in particular, the T-linear behavior in the strange metal (SM) and upper pseudogap (PG) phases, the pure $T^2$, Fermi liquid (FL) behavior observed in the strongly overdoped regime as well as the $T^{1+\delta}$ behavior that interpolates both in the crossover. We calculate the coefficients: a) of $T$ in the linear regime and show that it is proportional to the PG temperature $T^*(x)$; b) of the $T^2$-term in the FL regime, without adjusting any parameter; and c) of the $T^{1.6}$ term in the crossover regime, all in excellent agreement with the experimental data. From our model, we are able to infer that the resistivity in cuprates is caused by the scattering of holes by excitons, which naturally form as holes are doped into the electron background.",2004.12785v1 2012-01-05,Phonon-limited transport coefficients in extrinsic graphene,"The effect of electron-phonon scattering processes over the thermoelectric properties of extrinsic graphene was studied. Electrical and thermal resistivity, as well as the thermopower, were calculated within the Bloch theory approximations. Analytical expressions for the different transport coefficients were obtained from a variational solution of the Boltzmann equation. The phonon-limited electrical resistivity \rho_{e-ph} shows a linear dependence at high temperatures, and follows {\rho}_{e-ph} \sim T^{4} at low temperatures, in agreement with experiments and theory previously reported in the literature. The phonon-limited thermal resistivity at low temperatures exhibits a \sim T dependence, and achieves a nearly constant value at high temperatures. The predicted Seebeck coefficient at verylow temperatures is Q(T) \sim -\pi 2 k_B T /(3 e E_F), which shows a n^{-1/2} dependence with the density of carriers, in agreement with experimental evidence. Our results suggest that thermoelectric properties can be controlled by adjusting the Bloch-Gruneisen temperature through its dependence on the extrinsic carrier density in graphene.",1201.1057v1 2012-01-27,Giant negative magnetoresistance in high-mobility 2D electron systems,"We report on a giant negative magnetoresistance in very high mobility GaAs/AlGaAs heterostructures and quantum wells. The effect is the strongest at $B \simeq 1$ kG, where the magnetoresistivity develops a minimum emerging at $T \lesssim 2$ K. Unlike the zero-field resistivity which saturates at $T \simeq 2 $ K, the resistivity at this minimum continues to drop at an accelerated rate to much lower temperatures and becomes several times smaller than the zero-field resistivity. Unexpectedly, we also find that the effect is destroyed not only by increasing temperature but also by modest in-plane magnetic fields. The analysis shows that giant negative magnetoresistance cannot be explained by existing theories considering interaction-induced or disorder-induced corrections.",1201.5679v1 2019-03-12,DEM simulation of soil-tool interaction under extraterrestrial environmental effects,"In contrast to terrestrial environment, the harsh lunar environment conditions include lower gravity acceleration, ultra-high vacuum and high (low) temperature in the daytime (night-time). This paper focuses on the effects of those mentioned features on soil cutting tests, a simplified excavation test, to reduce the risk of lunar excavation missions. Soil behavior and blade performance were analyzed under different environmental conditions. The results show that: (1) the cutting resistance and the energy consumption increase linearly with the gravity. The bending moment has a bigger increasing rate in low gravity fields due to a decreasing moment arm; (2) the cutting resistance,energy consumption and bending moment increase significantly because of the raised soil strength on the lunar environment, especially in low gravity fields. Under the lunar environment, the proportions of cutting resistance, bending moment and energy consumption due to the effect of the van der Waals forces are significant. Thus, they should be taken into consideration when planning excavations on the Moon. Therefore, considering that the maximum frictional force between the excavator and the lunar surface is proportional to the gravity acceleration, the same excavator that works efficiently on the Earth may not be able to work properly on the Moon.",1903.04821v1 2019-04-05,Superconductivity in the dilute single band limit in reduced Strontium Titanate,"We report on superconductivity in single crystals of SrTiO$_{3-\delta}$ with carrier densities $\textit{n} < 1.4 \times10^{18}cm^{-3}$, where only a single band is occupied. For all samples in this regime, the resistive transition occurs at $T_{c} \approx 65 \pm 25 \ mK$. We observe a zero resistance state for $\textit{n}$ as low as $1.03 \times10^{17}cm^{-3}$, and a partial resistive transition for $\textit{n} = 3.85 \times10^{16}cm^{-3}$. We observe low critical current densities, relatively high and isotropic upper critical fields, and an absence of diamagnetic screening in these samples. Our findings suggest an inhomogeneous superconducting state, embedded within a homogeneous high-mobility 3-dimensional electron gas. $T_{c}$ does not vary appreciably when $\textit{n}$ changes by more than an order of magnitude, inconsistent with conventional superconductivity.",1904.03121v2 2012-06-25,A Study of Ni-Substitution Effects on Heavy-Fermion CeCu2Si2 - Similarities between Ni Substitution and High-Pressure Effects -,"The effects of Ni substitution on Ce(Cu1-xNix)2Si2 have been studied by specific heat and electrical resistivity measurements. The specific heat measurement has revealed that the enhanced quantum fluctuations around an antiferromagnetic quantum critical point are markedly suppressed by Ni substitution, and that the Fermi liquid state recovers in the Nirich region (x > 0.12). The characteristic T-linear dependence of the resistivity has been observed at approximately x ~ 0.10 together with a sign of superconductivity. The variation of n in the form of rho - rho0 = aT^n against Tmax^1, at which the resistivity peaks, coincides with the case of high-pressure experiments on pure CeCu2Si2. The anomalous T-linear behavior appears to occur in the crossover region from the Kondo regime to the valence fluctuation regime rather than in the conventional antiferromagnetic quantum critical region.",1206.5747v1 2015-07-08,Future Large-Scale Memristive Device Crossbar Arrays: Limits Imposed by Sneak-Path Currents on Read Operations,"Passive crossbar arrays based upon memristive devices, at crosspoints, hold great promise for the future high-density and non-volatile memories. The most significant challenge facing memristive device based crossbars today is the problem of sneak-path currents. In this paper, we investigate a memristive device with intrinsic rectification behavior to suppress the sneak-path currents in crossbar arrays. The device model is implemented in Verilog-A language and is simulated to match device characteristics readily available in the literature. Then, we systematically evaluate the read operation performance of large-scale crossbar arrays utilizing our proposed model in terms of read margin and power consumption while considering different crossbar sizes, interconnect resistance values, HRS/LRS (High Resistance State/Low Resistance State) values, rectification ratios and different read-schemes. The outcomes of this study are understanding the trade-offs among read margin, power consumption, read-schemes and most importantly providing a guideline for circuit designers to improve the performance of a memory based crossbar structure. In addition, read operation performance comparison of the intrinsic rectifying memristive device model with other memristive device models are studied.",1507.02077v1 2020-01-31,Dynamo in weakly collisional nonmagnetized plasmas impeded by Landau damping of magnetic fields,"We perform fully kinetic simulations of flows known to produce dynamo in magnetohydrodynamics (MHD), considering scenarios with low Reynolds number and high magnetic Prandtl number, relevant for galaxy cluster scale fluctuation dynamos. We find that Landau damping on the electrons leads to a rapid decay of magnetic perturbations, impeding the dynamo. This collisionless damping process operates on spatial scales where electrons are nonmagnetized, reducing the range of scales where the magnetic field grows in high magnetic Prandtl number fluctuation dynamos. When electrons are not magnetized down to the resistive scale, the magnetic energy spectrum is expected to be limited by the scale corresponding to magnetic Landau damping or, if smaller, the electron gyroradius scale, instead of the resistive scale. In simulations we thus observe decaying magnetic fields where resistive MHD would predict a dynamo.",2001.11929v2 2020-07-24,Strange Metallic Transport in the Antiferromagnetic Regime of Electron Doped Cuprates,"We report magnetoresistance and Hall Effect results for electron-doped films of the high-temperature superconductor La$_{2-x}$Ce$_x$CuO$_4$ (LCCO) for temperatures from 0.7 to 45 K and magnetic fields up to 65 T. For x = 0.12 and 0.13, just below the Fermi surface reconstruction (FSR), the normal state in-plane resistivity exhibits a well-known upturn at low temperature. Our new results show that this resistivity upturn is eliminated at high magnetic field and the resistivity becomes linear-in-temperature from $\sim$ 40 K down to 0.7 K. The magnitude of the linear coefficient scales with Tc and doping, as found previously [1,2] for dopings above the FSR. In addition, the normal state Hall coefficient has an unconventional field dependence for temperatures below 50K. This anomalous transport data presents a new challenge to theory and suggests that the strange metal normal state is also present in the antiferromagnetic regime.",2007.12765v1 2020-08-26,An 8-bit In Resistive Memory Computing Core with Regulated Passive Neuron and Bit Line Weight Mapping,"The rapid development of Artificial Intelligence (AI) and Internet of Things (IoT) increases the requirement for edge computing with low power and relatively high processing speed devices. The Computing-In-Memory(CIM) schemes based on emerging resistive Non-Volatile Memory(NVM) show great potential in reducing the power consumption for AI computing. However, the device inconsistency of the non-volatile memory may significantly degenerate the performance of the neural network. In this paper, we propose a low power Resistive RAM (RRAM) based CIM core to not only achieve high computing efficiency but also greatly enhance the robustness by bit line regulator and bit line weight mapping algorithm. The simulation results show that the power consumption of our proposed 8-bit CIM core is only 3.61mW (256*256). The SFDR and SNDR of the CIM core achieve 59.13 dB and 46.13 dB, respectively. The proposed bit line weight mapping scheme improves the top-1 accuracy by 2.46% and 3.47% for AlexNet and VGG16 on ImageNet Large Scale Visual Recognition Competition 2012 (ILSVRC 2012) in 8-bit mode, respectively.",2008.11669v1 2022-04-29,Nonlocal thermoelectric resistance in vortical viscous transport,"The pursuit for clearly identifiable signatures of viscous electron flow in the solid state systems has been a paramount task in the search of the hydrodynamic electron transport behavior. In this work, we investigate theoretically the nonlocal electric and thermal resistances for the generic non-Galilean-invariant electron liquids in the multiterminal Hall-bar devices in the hydrodynamic regime. The role of the device inhomogeneity is carefully addressed in the model of the disorder potential with the long-range correlation radius. We obtain analytic expressions for the thermoelectric resistances that are applicable in the full crossover regime from charge neutrality to high electron density. We show that the vortical component of the electron flow manifests in the thermal transport mode close to the charge neutrality where vorticity is already suppressed by the intrinsic conductivity in the electric current. This behavior can be tested by the high-resolution thermal imaging probes.",2204.14104v2 2022-11-04,In-plane anisotropy of electrical transport in Y$_{0.85}$Tb$_{0.15}$Ba$_2$Cu$_3$O$_{7-x}$ films,"We fabricate high-quality c-axis oriented epitaxial YBa$_2$Cu$_3$O$_{7-x}$ films with 15% of yttrium atoms replaced by terbium (YTBCO) and study their electrical properties. The Tb substitution reduces the charge carrier density resulting in increased resistivity and decreased critical current density compared to the pure YBa$_2$Cu$_3$O$_{7-x}$ films. The electrical properties of the YTBCO films show an in-plane anisotropy in both the superconducting and normal state providing evidence for the twin-free film. Unexpectedly, the resistive transition of the bridges also demonstrates the in-plane anisotropy that can be explained within the framework of Tinkham's model of the resistive transition and the Berezinskii-Kosterlitz-Thouless (BKT) model depending on the sample parameters. We consider YTBCO films to be a promising platform for both the fundamental research on the BKT transition in the cuprate superconductors and for the fabrication of devices with high kinetic inductance.",2211.02564v2 2023-02-23,Anomalous Electronic Transport in High Mobility Corbino Rings,"We report low-temperature electronic transport measurements performed in two multi-terminal Corbino samples formed in GaAs/Al-GaAs two-dimensional electron gases (2DEG) with both ultra-high electron mobility ($\gtrsim 20\times 10^6$ $cm^2/Vs)$ and with distinct electron density of $1.7$ and $3.6\times 10^{11}~cm^{-2}$. In both Corbino samples, a non-monotonic behavior is observed in the temperature dependence of the resistance below 1~$K$. Surprisingly, a sharp {\it decrease} in resistance is observed with {\it increasing} temperature in the sample with lower electron density, whereas an opposite behavior is observed in the sample with higher density. To investigate further, transport measurements were performed in large van der Pauw samples having identical heterostructures, and as expected they exhibit resistivity that is monotonic with temperature. Finally, we discuss the results in terms of various lengthscales leading to ballistic and hydrodynamic electronic transport, as well as a possible Gurzhi effect.",2302.12147v2 2024-01-01,"Debye temperature, electron-phonon coupling constant, and microcrystalline strain in highly-compressed La$_3$Ni$_2$O$_{7-δ}$","Recently Sun et al (Nature 621, 493 (2023)) reported on the discovery of high-temperature superconductivity in highly-compressed La$_3$Ni$_2$O$_{7-\delta}$. In addition to ongoing studies of the phase structural transition, pairing mechanism, and other properties/parameters in this highly-pressurized nickelate, here explore a possibility for the electron-phonon pairing mechanism in the La$_3$Ni$_2$O$_{7-\delta}$. To do this, we analyzed experimental data on temperature dependent resistance, $R(T)$, and extracted pressure dependent Debye temperature, $\Theta_D$, for the $Fmmm$-phase (high-pressure phase). Derived ballpark value is $\Theta_D(P = 25 GPa) = 550$ $K$. We also estimated the electron-phonon coupling constant, $\lambda_{e-ph}(P=22.4 GPa) = 1.75$, for La$_3$Ni$_2$O$_{7-\delta}$ sample exhibited zero-resistance transition. Performed analysis of XRD data showed that the crystal lattice strain, $\epsilon(P)$, is higher in the $Fmmm$-phase in comparison with the $Amam$-phase (low-pressure phase). Based on performed $\epsilon(P)$ analysis, we proposed possible reason for the presence/absence of the zero-resistance state in La$_3$Ni$_2$O$_{7-\delta}$.",2401.00804v2 2024-01-15,Comprehensive Joint Modeling of First-Line Therapeutics in Non-Small Cell Lung Cancer,"First-line antiproliferatives for non-small cell lung cancer (NSCLC) have a relatively high failure rate due to high intrinsic resistance rates and acquired resistance rates to therapy. 57% patients are diagnosed in late-stage disease due to the tendency of early-stage NSCLC to be asymptomatic. For patients first diagnosed with metastatic disease the 5-year survival rate is approximately 5%. To help accelerate the development of novel therapeutics and computer-based tools for optimizing individual therapy, we have collated data from 11 different clinical trials in NSCLC and developed a semi-mechanistic, clinical model of NSCLC growth and pharmacodynamics relative to the various therapeutics represented in the study. In this study, we have produced extremely precise estimates of clinical parameters fundamental to cancer modeling such as the rate of acquired resistance to various pharmaceuticals, the relationship between drug concentration and rate of cancer cell death, as well as the fine temporal dynamics of anti-VEGF therapy. In the simulation sets documented in this study, we have used the model to make meaningful descriptions of efficacy gain in making bevacizumab-antiproliferative combination therapy sequential, over a series of days, rather than concurrent.",2401.07719v1 2018-11-09,A Detailed Model of the Irish High Voltage Power Network for Simulating GICs,"Constructing a power network model for geomagnetically induced current (GIC) calculations requires information on the DC resistances of elements within a network. This information is often not known, and power network models are simplified as a result, with assumptions used for network element resistances. Ireland's relatively small, isolated network presents an opportunity to model a complete power network in detail, using as much real-world information as possible. A complete model of the Irish 400, 275, 220 and 110 kV network was made for GIC calculations, with detailed information on the number, type and DC resistances of transformers. The measured grounding resistances at a number of substations were also included in the model, which represents a considerable improvement on previous models of the Irish power network for GIC calculations. Sensitivity tests were performed to show how calculated GIC amplitudes are affected by different aspects of the model. These tests investigated: (1) How the orientation of a uniform electric field affects GICs. (2) The effect of including/omitting lower-voltage elements of the power network. (3) How the substation grounding resistances assumptions affected GIC values. It was found that changing the grounding resistance value had a considerable effect on calculated GICs at some substations, and no discernible effect at others. Finally, five recent geomagnetic storm events were simulated in the network. It was found that heavy rainfall prior to the 26-28 August 2015 geomagnetic storm event may have had a measurable impact on measured GIC amplitudes at a 400/220 kV transformer ground.",1811.04128v1 2020-03-09,Understanding the reduction of the edge safety factor during hot VDEs and fast edge cooling events,"In the present work a simple analytical approach is presented in order to clarify the physics behind the edge current density behaviour of a hot plasma entering in contact with a resistive conductor. When a plasma enters in contact with a highly resistive wall, large current densities appear at the edge of the plasma. The model shows that this edge current originates from the plasma response, which attempts to conserve the poloidal magnetic flux ($\Psi$) when the outer current is being lost. The loss of outer current is caused by the high resistance of the outer current path compared to the plasma core resistance. The resistance of the outer path may be given by plasma contact with a very resistive structure or by a sudden decrease of the outer plasma temperature (e.g. due to a partial thermal quench or due to a cold front penetration caused by massive gas injection). For general plasma geometries and current density profiles the model shows that given a small change of minor radius ($\delta a$) the plasma current is conserved to first order ($\delta I_p = 0 + \mathcal{O}(\delta a^2)$). This conservation comes from the fact that total inductance remains constant ($\delta L = 0$) due to an exact compensation of the change of external inductance with the change of internal inductance ($\delta L_\text{ext}+\delta L_\text{int} = 0$). As the total current is conserved and the plasma volume is reduced, the edge safety factor drops according to $q_a \propto a^2/I_p$. Finally the consistency of the resulting analytical predictions is checked with the help of free-boundary MHD simulations.",2003.04064v1 2019-07-24,GR-MHD disk winds and jets from black holes and resistive accretion disks,"We perform GR-MHD simulations of outflow launching from thin accretion disks. As in the non-relativistic case, resistivity is essential for the mass loading of the disk wind. We implemented resistivity in the ideal GR-MHD code HARM3D, extending previous works (Qian et al. 2017, 2018) for larger physical grids, higher spatial resolution, and longer simulation time. We consider an initially thin, resistive disk orbiting the black hole, threaded by a large-scale magnetic flux. As the system evolves, outflows are launched from the black hole magnetosphere and the disk surface. We mainly focus on disk outflows, investigating their MHD structure and energy output in comparison with the Poynting-dominated black hole jet. The disk wind encloses two components -- a fast component dominated by the toroidal magnetic field and a slower component dominated by the poloidal field. The disk wind transitions from sub to super-Alfv\'enic speed, reaching velocities $\simeq 0.1c$. We provide parameter studies varying spin parameter and resistivity level, and measure the respective mass and energy fluxes. A higher spin strengthens the $B_{\phi}$-dominated disk wind along the inner jet. We disentangle a critical resistivity level that leads to a maximum matter and energy output for both, resulting from the interplay between re-connection and diffusion, which in combination govern the magnetic flux and the mass loading. For counter-rotating black holes the outflow structure shows a magnetic field reversal. We estimate the opacity of the inner-most accretion stream and the outflow structure around it. This stream may be critically opaque for a lensed signal, while the axial jet funnel remains optically thin.",1907.10622v1 2017-05-23,The influence of outflow and global magnetic field on the structure and spectrum of resistive CDAFs,"We examine the effects of a global magnetic field and outflow on radiatively inefficient accretion flow (RIAF) in the presence of magnetic resistivity. We find a self-similar solutions for the height integrated equations that govern the behavior of the flow. We use the mixing length mechanism for studying the convection parameter. We adopt a radius dependent mass accretion rate as $\dot{M}=\dot{M}_{out}{(\frac{r}{r_{out}})^{s}}$ with $s> 0$ to investigate the influence of outflow on the structure of inflow where $s$ is a constant and indication the effect of wind. Also, we have studied the radiation spectrum and temperature of CDAFs. The thermal bermsstrahlung emission as a radiation mechanism is taken into account for calculating the spectra emitted by the CDAFs. The energy that powers bremsstrahlung emission at large radii is provided by convective transport from small radii and viscous and resistivity dissipation. Our results indicate that the disc rotates slower and accretes faster, it becomes hotter and thicker for stronger wind. By increasing all component of magnetic field, the disc rotates faster and accretes slower while it becomes hotter and thicker. We show that the outflow parameter and all component of magnetic field have the same effects on the luminosity of the disc. We compare the dynamical structure of the disc in two different solutions (with and without resistivity parameter). We show that only the radial infall velocity and the surface density could changed by resistivity parameter obviously. Increasing the effect of wind increases the disc's temperature and luminosity of the disc. The effect of magnetic field is similar to the effect of wind in the disc's temperature and luminosity of the disc, but the influence of resistivity on the observational properties is not evident.",1705.08099v1 2020-01-21,Particle acceleration with anomalous pitch angle scattering in 3D separator reconnection,"Understanding how the release of stored magnetic energy contributes to the generation of non-thermal high energy particles during solar flares is an important open problem in solar physics. Magnetic reconnection plays a fundamental role in the energy release and conversion processes taking place during flares. A common approach for investigating particle acceleration is to use test particles in fields derived from magnetohydrodynamic (MHD) simulations of reconnection. These MHD simulations use anomalous resistivities that are much larger than the Spitzer resistivity based on Coulomb collisions. The processes leading to enhanced resistivity should also affect the test particles. We explore the link between resistivity and particle orbits building on a previous study using a 2D MHD simulation of magnetic reconnection. This paper extends the previous investigation to a 3D magnetic reconnection configuration and to study the effect on test particle orbits. We carried out orbit calculations using a 3D MHD simulation of separator reconnection. We use the relativistic guiding centre approximation including stochastic pitch angle scattering. The effects of varying the resistivity and the models for pitch angle scattering on particle orbit trajectories, final positions, energy spectra, final pitch angle distribution, and orbit duration are all studied in detail. Pitch angle scattering widens collimated beams of orbit trajectories, allowing orbits to access previously unaccessible field lines; this causes final positions to spread to topological structures that were previously inaccessible. Scattered orbit energy spectra are found to be predominantly affected by the level of anomalous resistivity, with the pitch angle scattering model only playing a role in isolated cases. Scattering is found to play a crucial role in determining the pitch angle and orbit duration distributions.",2001.07548v1 2021-07-27,Resistance distance distribution in large sparse random graphs,"We consider an Erdos-Renyi random graph consisting of N vertices connected by randomly and independently drawing an edge between every pair of them with probability c/N so that at N->infinity one obtains a graph of finite mean degree c. In this regime, we study the distribution of resistance distances between the vertices of this graph and develop an auxiliary field representation for this quantity in the spirit of statistical field theory. Using this representation, a saddle point evaluation of the resistance distance distribution is possible at N->infinity in terms of an 1/c expansion. The leading order of this expansion captures the results of numerical simulations very well down to rather small values of c; for example, it recovers the empirical distribution at c=4 or 6 with an overlap of around 90%. At large values of c, the distribution tends to a Gaussian of mean 2/c and standard deviation sqrt{2/c^3}. At small values of c, the distribution is skewed toward larger values, as captured by our saddle point analysis, and many fine features appear in addition to the main peak, including subleading peaks that can be traced back to resistance distances between vertices of specific low degrees and the rest of the graph. We develop a more refined saddle point scheme that extracts the corresponding degree-differentiated resistance distance distributions. We then use this approach to recover analytically the most apparent of the subleading peaks that originates from vertices of degree 1. Rather intuitively, this subleading peak turns out to be a copy of the main peak, shifted by one unit of resistance distance and scaled down by the probability for a vertex to have degree 1. We comment on a possible lack of smoothness in the true N->infinity distribution suggested by the numerics.",2107.12561v2 2002-01-30,Activity in Very Cool Stars: Magnetic Dissipation in late-M and L Dwarf Atmospheres,"Recent observations show that chromospheric activity in late-M and L dwarfs is much lower than in the earlier M types, in spite of comparatively rapid rotation. We investigate the possibility that this drop-off in activity results from the very high electrical resistivities in the dense, cool and predominantly neutral atmospheres of late-M and L dwarfs. We calculate magnetic field diffusivities in the atmospheres of objects with effective temperatures in the range 3000-1500 (mid-M to L), using the atmospheric structure models of Allard and Hauschildt. We find that the combination of very low ionization fraction and high density in these atmospheres results in very large resistivities due to neutral-charged particle collisions, and efficient field diffusion. The resistivities are found to increase with both decreasing optical depth, and decreasing effective temperature. As a result, any existing magnetic fields are increasingly decoupled from atmospheric motions as one moves from mid-M to L; we quantify this through a simple Reynolds number calculation. This, coupled with the difficulty in transporting magnetic stresses through the highly resistive atmosphere, can account for the observed drop in activity from mid-M to L, assuming activity in these objects is magnetically driven. We also examine the issue of acoustic heating, and find that this appears inadequate to explain the observed H-alpha fluxes in mid-M to L dwarfs. Consequently, magnetic heating does seem to be the most viable mechanism for generating activity in these objects. Finally, we speculate on a possible flare mechanism in these cool dwarfs.",0201518v1 1996-11-14,Vortex Quantum Nucleation and Tunneling in Superconducting Thin Films: Role of Dissipation and Periodic Pinning,"We investigate the phenomenon of decay of a supercurrent in a superconducting thin film in the absence of an applied magnetic field. The resulting zero-temperature resistance derives from two equally possible mechanisms: 1) quantum tunneling of vortices from the edges of the sample; and 2) homogeneous quantum nucleation of vortex-antivortex pairs in the bulk of the sample, arising from the instability of the Magnus field's ``vacuum''. We study both situations in the case where quantum dissipation dominates over the inertia of the vortices. We find that the vortex tunneling and nucleation rates have a very rapid dependence on the current density driven through the sample. Accordingly, whilst normally the superconductor is essentially resistance-free, for the high current densities that can be reached in high-$T_c$ films a measurable resistance might develop. We show that edge-tunneling appears favoured, but the presence of pinning centres and of thermal fluctuations leads to an enhancement of the nucleation rates. In the case where a periodic pinning potential is artificially introduced in the sample, we show that current-oscillations will develop indicating an effect specific to the nucleation mechanism where the vortex pair-production rate, thus the resistance, becomes sensitive to the corrugation of the pinning substrate. In all situations, we give estimates for the observability of the studied phenomena.",9611112v1 1997-12-19,C-axis resistivity and high Tc superconductivity,"Recently we had proposed a mechanism for the normal-state C-axis resistivity of the high-T$_c$ layered cuprates that involved blocking of the single-particle tunneling between the weakly coupled planes by strong intra-planar electron-electron scattering. This gave a C-axis resistivity that tracks the ab-plane T-linear resistivity, as observed in the high-temperature limit. In this work this mechanism is examined further for its implication for the ground-state energy and superconductivity of the layered cuprates. It is now argued that, unlike the single-particle tunneling, the tunneling of a boson-like pair between the planes prepared in the BCS-type coherent trial state remains unblocked inasmuch as the latter is by construction an eigenstate of the pair annihilation operator. The resulting pair-delocalization along the C-axis offers energetically a comparative advantage to the paired-up trial state, and, thus stabilizes superconductivity. In this scheme the strongly correlated nature of the layered system enters only through the blocking effect, namely that a given electron is effectively repeatedly monitored (intra-planarly scattered) by the other electrons acting as an environment, on a time-scale shorter than the inter-planar tunneling time. Possible relationship to other inter-layer pairing mechanisms proposed by several workers in the field is also briefly discussed.",9712247v2 2000-07-03,Electron-Phonon Coupling Origin of the resistivity in YNi_{2}B_{2}C Single Crystals,"Resistivity measurements from 4.2 K up to 300 K were made on YNi_{2}B_{2}C single crystals with Tc=15.5 K. The resulting rho(T) curve shows a perfect Bloch-Grueneisen (BG) behavior, with a very small residual resistivity which indicates the low impurity content and the high cristallographic quality of the samples. The value lambda_{tr}=0.53 for the transport electron-phonon coupling constant was obtained by using the high-temperature constant value of d(rho)/dT and the plasma frequency reported in literature. The BG expression for the phononic part of the resistivity rho_{ph}(T) was then used to fit the data in the whole temperature range, by approximating alpha^{2}_{tr}F(Omega) with the experimental phonon spectral density G(Omega) multiplied by a two-step weighting function to be determined by the fit. The resulting fitting curve perfectly agrees with the experimental points. We also solved the real-axis Eliashberg equations in both s- and d-wave symmetries under the approximation alpha^{2}F(Omega)= alpha^{2}_{tr}F(Omega). We found that the value of lambda_{tr} here determined in single-band approximation is quite compatible with Tc and the gap Delta experimentally observed. Finally, we calculated the normalized tunneling conductance, whose comparison with break-junction tunnel data gives indication of the possible s-wave symmetry for the order parameter in YNi_{2}B_{2}C.",0007033v1 2010-12-10,High pressure study of transport properties in Co$_{1/3}$NbS$_2$,"This is the first study of the effect of pressure on transition metal dichalcogenides intercalated by atoms that order magnetically. Co$_{1/3}$NbS$_2$ is a layered system where the intercalated Co atoms order antiferromagnetically at T$_N$ = 26 K at ambient pressure. We have conducted a detailed study of dc-resistivity ($\rho$), thermoelectric power (S) and thermal conductivity ($\kappa$). We found that at ambient pressure the magnetic transition corresponds to a well pronounced peak in dS/dT, as well as to a kink in the dc-resistivity. The effect of ordering on the thermal conductivity is rather small but, surprisingly, more pronounced in the lattice contribution than in the electronic contribution to $\kappa$. Under pressure, the resistivity increases in the high temperature range, contrary to all previous measurements in other layered transition metal dichalcogenides (TMD). In the low temperature range, the strong dependences of thermopower and resistivity on pressure are observed below TN, which, in turn, also depends on pressure at rate of dT$_N$/dp $\approx$ -1 K/kbar. Several possible microscopic explanations of the reduction of the ordering temperature and the evolution of the transport properties with pressure are discussed.",1012.2408v1 2011-09-14,Evidence for a fractional quantum Hall state with anisotropic longitudinal transport,"At high magnetic fields, where the Fermi level lies in the N=0 lowest Landau level (LL), a clean two-dimensional electron system (2DES) exhibits numerous incompressible liquid phases which display the fractional quantized Hall effect (FQHE) (Das Sarma and Pinczuk, 1997). These liquid phases do not break rotational symmetry, exhibiting resistivities which are isotropic in the plane. In contrast, at lower fields, when the Fermi level lies in the $N\ge2$ third and several higher LLs, the 2DES displays a distinctly different class of collective states. In particular, near half filling of these high LLs the 2DES exhibits a strongly anisotropic longitudinal resistance at low temperatures (Lilly et al., 1999; Du et al., 1999). These ""stripe"" phases, which do not exhibit the quantized Hall effect, resemble nematic liquid crystals, possessing broken rotational symmetry and orientational order (Koulakov et al., 1996; Fogler et al., 1996; Moessner and Chalker, 1996; Fradkin and Kivelson, 1999; Fradkin et al, 2010). Here we report a surprising new observation: An electronic configuration in the N=1 second LL whose resistivity tensor simultaneously displays a robust fractionally quantized Hall plateau and a strongly anisotropic longitudinal resistance resembling that of the stripe phases.",1109.3219v3 2011-10-18,A numerical model of resistive generation of intergalactic magnetic field at cosmic dawn,"Miniati and Bell (2011) proposed a mechanism for the generation of magnetic seeds that is based the finite resistivity of the low temperature IGM in the high redshift universe. In this model, cosmic-ray protons generated by the first generation of galaxies, escape into the intergalactic medium carrying an electric current that induces return currents, $j_t$, and associated electric fields, $\vec E=\eta\vec j_t$ there. Because the resistivity, $\eta$, depends on the IGM temperature, which is highly inhomogeneous due to adiabatic contraction and shocks produced by structure formation, a non-vanishing curl of the electric field exists which sustains the growth of magnetic field. In this contribution we have developed an approximate numerical model for this process by implementing the source terms of the resistive mechanism in the cosmological code CHARM. Our numerical estimates substantiate the earlier analysis in Miniati and Bell (2011) which found magnetic seeds between 10$^{-18}$ and 10$^{-16}$ Gauss throughout cosmic space at redshift z~6, consistent with conservative estimates of magnetic fields in voids at z~0 from recent gamma-ray experiments.",1110.4115v1 2017-02-18,Soft-proton exchange on Magnesium-oxide-doped substrates a route toward efficient and power-resistant nonlinear converters,"Despite its attractive features, Congruent-melted Lithium Niobate (CLN) suffers from Photo-Refractive Damage (PRD). This light-induced refractive-index change hampers the use of CLN when high-power densities are in play, a typical regime in integrated optics. The resistance to PRD can be largely improved by doping the lithium-niobate substrates with magnesium oxide. However, the fabrication of waveguides on MgO-doped substrates is not as effective as for CLN: either the resistance to PRD is strongly reduced by the waveguide fabrication process (as it happens in Ti-indiffused waveguides) or the nonlinear conversion efficiency is lowered (as it occurs in annealed-proton exchange). Here we fabricate, for the first time, waveguides starting from MgO-doped substrates using the Soft-Proton Exchange (SPE) technique and we show that this third way represents a promising alternative. We demonstrate that SPE allows to produce refractive-index profiles almost identical to those produced on CLN without reducing the nonlinearity in the substrate. We also prove that the SPE does not affect substantially the resistance to PRD. Since the fabrication recipe is identical between CLN and MgO-doped substrates, we believe that SPE might outperform standard techniques to fabricate robust and efficient waveguides for high-intensity-beam confinement.",1702.05590v1 2019-04-11,Novel Resistive-Plate WELL sampling element for (S)DHCAL,"Digital and Semi-Digital Hadronic Calorimeters (S)DHCAL were suggested for future Colliders as part of the particle-flow concept. Though studied mostly with RPC-based techniques, investigations have shown that MPGD-based sampling elements could outperform. An attractive, industry-produced, robust, particle-tracking detector for large-area coverage, e.g. in (S)DHCAL, could be the novel single-stage Resistive Plate WELL (RPWELL). It is a single-sided THGEM coupled to the segmented readout electrode through a sheet of large bulk resistivity. We summarize here the preliminary test-beam results obtained with 6.5 mm thick (incl. electronics) {$48 \times 48\,\mathrm{cm^2}$}~RPWELL detectors. Two configurations are considered: a standalone RPWELL detector studied with 150 GeV muons and high-rate pions beams and RPWELL sampling element investigated within a small-(S)DHCAL prototype consisting of 7 resistive MICROMEGAS sampling elements followed by 5 RPWELL ones. The sampling elements were equipped with a Semi-Digital readout electronics based on the MICROROC chip.",1904.05545v2 2020-05-22,Accelerating Antimicrobial Discovery with Controllable Deep Generative Models and Molecular Dynamics,"De novo therapeutic design is challenged by a vast chemical repertoire and multiple constraints, e.g., high broad-spectrum potency and low toxicity. We propose CLaSS (Controlled Latent attribute Space Sampling) - an efficient computational method for attribute-controlled generation of molecules, which leverages guidance from classifiers trained on an informative latent space of molecules modeled using a deep generative autoencoder. We screen the generated molecules for additional key attributes by using deep learning classifiers in conjunction with novel features derived from atomistic simulations. The proposed approach is demonstrated for designing non-toxic antimicrobial peptides (AMPs) with strong broad-spectrum potency, which are emerging drug candidates for tackling antibiotic resistance. Synthesis and testing of only twenty designed sequences identified two novel and minimalist AMPs with high potency against diverse Gram-positive and Gram-negative pathogens, including one multidrug-resistant and one antibiotic-resistant K. pneumoniae, via membrane pore formation. Both antimicrobials exhibit low in vitro and in vivo toxicity and mitigate the onset of drug resistance. The proposed approach thus presents a viable path for faster and efficient discovery of potent and selective broad-spectrum antimicrobials.",2005.11248v2 2020-10-22,Projecting the optimal control strategy on invasive plants combining effects of herbivores and native plants resistance,"Understanding how to limit biological invasion is critical, especially in the context of accelerating anthropogenic ecological changes. Although biological invasion success could be explained by the lack of natural enemies in new regions, recent studies have revealed that resident herbivores often do have a substantial effect on both native and invasive plants. Very few studies have included consideration of native plant resistance while estimating methods of controlling invasion; hence, it is unclear to what extent the interactive effects of controlling approaches and native plants' resistance could slow down or even inhibit biological invasion. We developed a spatial modeling framework, using a paired logistic equation model, with considerations of the dispersal processes, to capture the dynamics change of native and invasive plants under various strategies of control. We found that when biocontrol agents could have a strong effect on invasive plant, that could almost completely limit the invasion, together with a high native plant resistance. However, a high application frequency is needed make an efficient impact, whereas, a low frequency treatment leads to nearly the same outcome as the no treatment case. Lastly, we showed that evenly controlling a larger area with a weaker effect still lead to a better outcome than focusing on small patches with a stronger effect. Overall, this study has some management implications, such as how to determine the optimal allocation strategy.",2010.14944v1 2021-10-14,Mitigation of parasitic losses in the quadrupole resonator enabling direct measurements of low residual resistances of SRF samples,"The quadrupole resonator (QPR) is a dedicated sample-test cavity for the RF characterization of superconducting samples in a wide temperature, RF field and frequency range. Its main purpose are high resolution measurements of the surface resistance with direct access to the residual resistance thanks to the low frequency of the first operating quadrupole mode. Besides the well-known high resolution of the QPR, a bias of measurement data towards higher values has been observed, especially at higher harmonic quadrupole modes. Numerical studies show that this can be explained by parasitic RF losses on the adapter flange used to mount samples into the QPR. Coating several micrometer of niobium on those surfaces of the stainless steel flange that are exposed to the RF fields significantly reduced this bias, enabling a direct measurement of a residual resistance smaller than 5 n$\Omega$ at 2 K and 413 MHz. A constant correction based on simulations was not feasible due to deviations from one measurement to another. However, this issue is resolved given these new results.",2110.07236v2 2022-01-27,On the Mitigation of Read Disturbances in Neuromorphic Inference Hardware,"Non-Volatile Memory (NVM) cells are used in neuromorphic hardware to store model parameters, which are programmed as resistance states. NVMs suffer from the read disturb issue, where the programmed resistance state drifts upon repeated access of a cell during inference. Resistance drifts can lower the inference accuracy. To address this, it is necessary to periodically reprogram model parameters (a high overhead operation). We study read disturb failures of an NVM cell. Our analysis show both a strong dependency on model characteristics such as synaptic activation and criticality, and on the voltage used to read resistance states during inference. We propose a system software framework to incorporate such dependencies in programming model parameters on NVM cells of a neuromorphic hardware. Our framework consists of a convex optimization formulation which aims to implement synaptic weights that have more activations and are critical, i.e., those that have high impact on accuracy on NVM cells that are exposed to lower voltages during inference. In this way, we increase the time interval between two consecutive reprogramming of model parameters. We evaluate our system software with many emerging inference models on a neuromorphic hardware simulator and show a significant reduction in the system overhead.",2201.11527v1 2024-03-20,Picosecond Femtojoule Resistive Switching in Nanoscale VO$_{2}$ Memristors,"Beyond-Moore computing technologies are expected to provide a sustainable alternative to the von Neumann approach not only due to their down-scaling potential but also via exploiting device-level functional complexity at the lowest possible energy consumption. The dynamics of the Mott transition in correlated electron oxides, such as vanadium dioxide, has been identified as a rich and reliable source of such functional complexity. However, its full potential in high-speed and low-power operation has been largely unexplored. We fabricated nanoscale VO$_{2}$ devices embedded in a broad-band test circuit to study the speed and energy limitations of their resistive switching operation. Our picosecond time-resolution, real-time resistive switching experiments and numerical simulations demonstrate that tunable low-resistance states can be set by the application of 20~ps long, $<$1.7~V amplitude voltage pulses at 15~ps incubation times and switching energies starting from a few femtojoule. Moreover, we demonstrate that at nanometer-scale device sizes not only the electric field induced insulator-to-metal transition, but also the thermal conduction limited metal-to-insulator transition can take place at timescales of 100's of picoseconds. These orders of magnitude breakthroughs open the route to the design of high-speed and low-power dynamical circuits for a plethora of neuromorphic computing applications from pattern recognition to numerical optimization.",2403.13530v1 2024-05-21,A lightweight PUF-based authentication protocol,"Lightweight authentication is essential for resource-constrained Internet-of-Things (IoT). Implementable with low resource and operable with low power, Physical Unclonable Functions (PUFs) have the potential as hardware primitives for implementing lightweight authentication protocols. The arbiter PUF (APUF) is probably the most lightweight strong PUF capable of generating exponentially many challenge-response pairs (CRPs), a desirable property for authentication protocols, but APUF is severely weak against modeling attacks. Efforts on PUF design have led to many PUFs of higher resistance to modeling attacks and also higher area overhead. There are also substantial efforts on protocol development, some leverage PUFs' strength in fighting modeling attacks, and some others employ carefully designed protocol techniques to obfuscate either the challenges or the responses with modest increase of area overhead for some or increased operations for some others. To attain both low resource footprint and high modeling attack resistance, in this paper we propose a co-design of PUF and protocol, where the PUF consists of an APUF and a zero-transistor interface that obfuscates the true challenge bits fed to the PUF. The obfuscated PUF possesses rigorously proven potential and experimentally supported performance against modeling attacks when a condition is met, and the protocol provides the condition required by the PUF and leverages the PUF's modeling resistance to arrive at low resource overhead and high operational simplicity, enabling lightweight authentications while resisting modeling attacks.",2405.13146v1 2008-04-14,Phase Diagram and Quantum Critical Point in Newly Discovered Superconductors: SmO_{1-x}F_xFeAs,"The magnetic fluctuations associated with a quantum critical point (QCP) are widely believed to cause the non-Fermi liquid behaviors and unconventional superconductivities, for example, in heavy fermion systems and high temperature cuprate superconductors. Recently, superconductivity has been discovered in iron-based layered compound $LaO_{1-x}F_xFeAs$ with $T_c$=26 K\cite{yoichi}, and it competes with spin-density-wave (SDW) order\cite{dong}. Neutron diffraction shows a long-rang SDW-type antiferromagnetic (AF) order at $\sim 134$ K in LaOFeAs\cite{cruz,mcguire}. Therefore, a possible QCP and its role in this system are of great interests. Here we report the detailed phase diagram and anomalous transport properties of the new high-Tc superconductors $SmO_{1-x}F_xFeAs$ discovered by us\cite{chenxh}. It is found that superconductivity emerges at $x\sim$0.07, and optimal doping takes place in the $x\sim$0.20 sample with highest $T_c \sim $54 K. While $T_c$ increases monotonically with doping, the SDW order is rapidly suppressed, suggesting a QCP around $x \sim$0.14. As manifestations, a linear temperature dependence of the resistivity shows up at high temperatures in the $x<0.14$ regime, but at low temperatures just above $T_c$ in the $x>0.14$ regime; a drop in carrier density evidenced by a pronounced rise in Hall coefficient are observed, which mimic the high-$T_c$ cuprates. The simultaneous occurrence of order, carrier density change and criticality makes a compelling case for a quantum critical point in this system.",0804.2105v3 2008-07-07,Magnetoresistance and collective Coulomb blockade in super-lattices of ferromagnetic CoFe nanoparticles,"We report on transport properties of millimetric super-lattices of CoFe nanoparticles surrounded by organic ligands. R(T)s follow R(T) = R_0.exp(T/T_0)^0.5 with T_0 ranging from 13 to 256 K. At low temperature I(V)s follow I=K[(V-V_T)/V_T]^ksi with ksi ranging 3.5 to 5.2. I(V) superpose on a universal curve when shifted by a voltage proportional to the temperature. Between 1.8 and 10 K a high-field magnetoresistance with large amplitude and a strong voltage-dependence is observed. Its amplitude only depends on the magnetic field/temperature ratio. Its origin is attributed to the presence of paramagnetic states present at the surface or between the nanoparticles. Below 1.8 K, this high-field magnetoresistance abruptly disappears and inverse tunnelling magnetoresistance is observed, the amplitude of which does not exceed 1%. At this low temperature, some samples display in their I(V) characteristics abrupt and hysteretic transitions between the Coulomb blockade regime and the conductive regime. The increase of the current during these transitions can be as high as a factor 30. The electrical noise increases when the sample is near the transition. The application of a magnetic field decreases the voltage at which these transitions occur so magnetic-field induced transitions are also observed. Depending on the applied voltage, the temperature and the amplitude of the magnetic field, the magnetic-field induced transitions are either reversible or irreversible. These abrupt and hysteretic transitions are also observed in resistance-temperature measurements. They could be the soliton avalanches predicted by Sverdlov et al. [Phys. Rev. B 64, 041302 (R), 2001] or could also be interpreted as a true phase transition between a Coulomb glass phase to a liquid phase of electrons.",0807.1060v3 2015-09-29,Simulation of radiation-induced defects,"Mainly due to their outstanding performance the position sensitive silicon detectors are widely used in the tracking systems of High Energy Physics experiments such as the ALICE, ATLAS, CMS and LHCb at LHC, the world's largest particle physics accelerator at CERN, Geneva. The foreseen upgrade of the LHC to its high luminosity (HL) phase (HL-LHC scheduled for 2023), will enable the use of maximal physics potential of the facility. After 10 years of operation the expected fluence will expose the tracking systems at HL-LHC to a radiation environment that is beyond the capacity of the present system design. Thus, for the required upgrade of the all-silicon central trackers extensive measurements and simulation studies for silicon sensors of different designs and materials with sufficient radiation tolerance have been initiated within the RD50 Collaboration. Supplementing measurements, simulations are in vital role for e.g. device structure optimization or predicting the electric fields and trapping in the silicon sensors. The main objective of the device simulations in the RD50 Collaboration is to develop an approach to model and predict the performance of the irradiated silicon detectors using professional software. The first successfully developed quantitative models for radiation damage, based on two effective midgap levels, are able to reproduce the experimentally observed detector characteristics like leakage current, full depletion voltage and charge collection efficiency (CCE). Recent implementations of additional traps at the SiO$_2$/Si interface or close to it have expanded the scope of the experimentally agreeing simulations to such surface properties as the interstrip resistance and capacitance, and the position dependency of CCE for strip sensors irradiated up to $\sim$$1.5\times10^{15}$ n$_{\textrm{eq}}\textrm{cm}^{-2}$.",1509.08657v1 2015-10-14,"Elastic Composite, Reinforced Lightweight Concrete as a Type of Resilient Composite Systems",". A kind of ""Elastic Composite, Reinforced Lightweight Concrete (ECRLC)"" with the mentioned specifics is a type of ""Resilient Composite Systems (RCS)"" in which, contrary to the basic geometrical assumption of flexure theory in Solid Mechanics, ""the strain changes in the beam height during bending"" is typically ""Non-linear"". . Through employing this integrated structure, with significant high strain capability and modulus of resilience in bending, we could constructively achieve high bearing capacities in beams with secure fracture pattern, in less weight. . Due to the system particulars and its behavior in bending, the usual calculation of the equilibrium steel amount to attain the low-steel bending sections with secure fracture pattern in the beams and its related limitations do not become propounded. Thereby, the strategic deadlock of high possibility of brittle fracture pattern in the bending elements made of the usual reinforced lightweight concretes, especially about the low-thickness bending elements as slabs, is being unlocked. . This simple, applied technology and the related components and systems can have several applications in ""the Road and Building Industries"" too. . Regarding the ""strategic importance of the Lightweight & Integrated Construction in practical increase of the resistance and safety against earthquake"" and considering the appropriate behavior of this resilient structure against the dynamic loads, shakes, impacts and shocks and capability of making some lightweight and insulating, non-brittle, reinforced sandwich panels and pieces, this system and its components could be also useful in ""seismic areas"". . This system could be also employed in constructing the vibration and impact absorber bearing pieces and slabs, which can be used in ""the Railroad & Subway Structures"" too. . Here, the ""RCS"" and ""ECRLC"" (as a type of RCS) have been concisely presented.",1510.03933v1 2018-01-26,Enhanced moments of Eu in single crystals of the metallic helical antiferromagnet EuCo{2-y}As2,"The compound EuCo{2-y}As2 with the tetragonal ThCr2Si2 structure is known to contain Eu{+2} ions with spin S = 7/2 that order below a temperature TN = 47 K into an antiferromagnetic (AFM) proper helical structure with the ordered moments aligned in the tetragonal ab plane, perpendicular to the helix axis along the c axis, with no contribution from the Co atoms. Here we carry out a detailed investigation of the properties of single crystals. Enhanced ordered and effective moments of the Eu spins are found in most of our crystals. Electronic structure calculations indicate that the enhanced moments arise from polarization of the d bands, as occurs in ferromagnetic Gd metal. Electrical resistivity measurements indicate metallic behavior. The low-field in-plane magnetic susceptibilities chi{ab}(T < TN) for several crystals are reported that are fitted well by unified molecular field theory (MFT), and the Eu-Eu exchange interactions Jij are extracted from the fits. High-field magnetization M data for magnetic fields H||ab reveal what appears to be a first-order spin-flop transition followed at higher field by a second-order metamagnetic transition of unknown origin, and then by another second-order transition to the paramagnetic (PM) state. For H||c, the magnetization shows only a second-order transition from the canted AFM to the PM state, as expected. The critical fields for the AFM to PM transition are in approximate agreement with the predictions of MFT. Heat capacity Cp measurements in zero and high H are reported. Phase diagrams for H||c and H||ab versus T are constructed from the high-field M(H,T) and Cp(H,T) measurements. The magnetic part Cmag(T, H = 0) of Cp(T, H = 0) is extracted and is fitted rather well below TN by MFT, although dynamic short-range AFM order is apparent in Cmag(T) up to about 70 K, where the molar entropy attains its high-T limit of R ln8.",1801.08941v1 2018-09-10,High-performance InSe Transistors with Ohmic Contact Enabled by Nonrectifying-barrier-type Indium Electrodes,"The electrical contact to two-dimensional (2D)-semiconductor materials are decisive to the electronic performance of 2D-semiconductor field-effect devices (FEDs). The presence of a Schottky barrier often leads to a large contact resistance, which seriously limits the channel conductance and carrier mobility measured in a two-terminal geometry. In contrast, ohmic contact is desirable and can be achieved by the presence of a nonrectifying or tunneling barrier. Here, we demonstrate that an nonrectifying barrier can be realized by contacting indium (In), a low work function metal, with layered InSe because of a favorable band alignment at the In-InSe interface. The nonrectifying barrier is manifested by ohmic contact behavior at T=2 K and a low barrier height, {\Phi}$_B$=50 meV. This ohmic contact enables demonstration of an ON-current as large as 410 {\mu}A/{\mu}m, which is among the highest values achieved in FEDs based on layered semiconductors. A high electron mobility of 3,700 and 1,000 cm$^2$/Vs is achieved with the two-terminal In-InSe FEDs at T=2 K and room temperature, respectively, which can be attributed to enhanced quality of both conduction channel and the contacts. The improvement in the contact quality is further proven by an X-ray photoelectron spectroscopy study, which suggests that a reduction effect occurs at the In-InSe interface. The demonstration of high-performance In-InSe FEDs indicates a viable interface engineering method for next-generation, 2D-semiconductor-based electronics.",1809.03181v1 2018-11-19,Characterisation of AMS H35 HV-CMOS monolithic active pixel sensor prototypes for HEP applications,"Monolithic active pixel sensors produced in High Voltage CMOS (HV-CMOS) technology are being considered for High Energy Physics applications due to the ease of production and the reduced costs. Such technology is especially appealing when large areas to be covered and material budget are concerned. This is the case of the outermost pixel layers of the future ATLAS tracking detector for the HL-LHC. For experiments at hadron colliders, radiation hardness is a key requirement which is not fulfilled by standard CMOS sensor designs that collect charge by diffusion. This issue has been addressed by depleted active pixel sensors in which electronics are embedded into a large deep implantation ensuring uniform charge collection by drift. Very first small prototypes of hybrid depleted active pixel sensors have already shown a radiation hardness compatible with the ATLAS requirements. Nevertheless, to compete with the present hybrid solutions a further reduction in costs achievable by a fully monolithic design is desirable. The H35DEMO is a large electrode full reticle demonstrator chip produced in AMS 350 nm HV-CMOS technology by the collaboration of Karlsruher Institut f\""ur Technologie (KIT), Institut de F\'isica d'Altes Energies (IFAE), University of Liverpool and University of Geneva. It includes two large monolithic pixel matrices which can be operated standalone. One of these two matrices has been characterised at beam test before and after irradiation with protons and neutrons. Results demonstrated the feasibility of producing radiation hard large area fully monolithic pixel sensors in HV-CMOS technology. H35DEMO chips with a substrate resistivity of 200$\Omega$ cm irradiated with neutrons showed a radiation hardness up to a fluence of $10^{15}$n$_{eq}$cm$^{-2}$ with a hit efficiency of about 99% and a noise occupancy lower than $10^{-6}$ hits in a LHC bunch crossing of 25ns at 150V.",1811.07817v3 2019-05-10,Vacuum electrical breakdown conditioning study in a parallel plate electrode pulsed DC system,"Conditioning of a metal structure in a high-voltage system is the progressive development of resistance to vacuum arcing over the operational life of the system. This is, for instance, seen during the initial operation of radio frequency (rf) cavities in particle accelerators. It is a relevant topic for any technology where breakdown limits performance, and where conditioning continues for a significant duration of system runtime. Projected future linear accelerators require structures with accelerating gradients of up to 100 MV/m. Currently, this performance level is only achievable after a multi-month conditioning period. In this work, a pulsed DC system applying voltage pulses over parallel disk electrodes was used to study the conditioning process, with the objective of obtaining insight into its underlying mechanics, and ultimately, to find ways to shorten the conditioning process. Two kinds of copper electrodes were tested: As-prepared machine-turned electrodes (""hard"" copper), and electrodes that additionally had been subjected to high temperature treatments (""soft"" copper). The conditioning behaviour of the soft electrodes was found to be similar to that of comparably treated accelerating structures, indicating a similar conditioning process. The hard electrodes reached the same ultimate performance as the soft electrodes much faster, with a difference of more than an order of magnitude in the number of applied voltage pulses. Two distinctly different distributions of breakdown locations were observed on the two types of electrodes. Considered together, our results support the crystal structure dislocation theory of breakdown, and suggest that the conditioning of copper in high field systems such as rf accelerating structures is dominated by material hardening.",1905.03996v1 2019-07-18,High-performance silicon-graphene hybrid plasmonic waveguide photodetectors beyond 1.55 μm,"A fast silicon-graphene hybrid plasmonic waveguide photodetectors beyond 1.55 {\mu}m is proposed and realized by introducing an ultra-thin wide silicon-on-insulator ridge core region with a narrow metal cap. With this novel design, the light absorption in graphene is enhanced while the metal absorption loss is reduced simultaneously, which helps greatly improve the responsivity as well as shorten the absorption region for achieving fast responses. Furthermore, metal-graphene-metal sandwiched electrodes are introduced to reduce the metal-graphene contact resistance, which is also helpful for improving the response speed. When the photodetector operates at 2 {\mu}m, the measured 3dB-bandwidth is >20 GHz (which is limited by the experimental setup) while the 3dB-bandwith calculated from the equivalent circuit with the parameters extracted from the measured S11 is as high as ~100 GHz. To the best of our knowledge, it is the first time to report the waveguide photodetector at 2 {\mu}m with a 3dB-bandwidth over 20 GHz. Besides, the present photodetectors also work very well at 1.55 {\mu}m. The measured responsivity is about 0.4 A/W under a bias voltage of -0.3 V for an optical power of 0.16 mW, while the measured 3dB-bandwidth is over 40 GHz (limited by the test setup) and the 3 dB-bandwidth estimated from the equivalent circuit is also as high as ~100 GHz, which is one of the best results reported for silicon-graphene photodetectors at 1.55 {\mu}m.",1907.12498v1 2020-07-01,Predicting Oxidation and Spin States by High-Dimensional Neural Networks: Applications to Lithium Manganese Oxide Spinels,"Lithium ion batteries often contain transition metal oxides like Li$_{x}$Mn$_2$O$_4$ ($0\leq x\leq2$). Depending on the Li content different ratios of Mn$^\text{III}$ to Mn$^\text{IV}$ ions are present. In combination with electron hopping the Jahn-Teller distortions of the Mn$^\text{III}$O$_6$ octahedra can give rise to complex phenomena like structural transitions and conductance. While for small model systems oxidation and spin states can be determined using density functional theory (DFT), the investigation of dynamical phenomena by DFT is too demanding. Previously, we have shown that a high-dimensional neural network potential can extend molecular dynamics (MD) simulations of Li$_{x}$Mn$_2$O$_4$ to nanosecond time scales, but these simulations did not provide information about the electronic structure. Here we extend the use of neural networks to the prediction of atomic oxidation and spin states. The resulting high-dimensional neural network is able to predict the spins of the Mn ions with an error of only 0.03 $\hbar$. We find that the Mn e$_\text{g}$ electrons are correctly conserved and that the number of Jahn-Teller distorted Mn$^\text{III}$O$_6$ octahedra is predicted precisely for different Li loadings. A charge ordering transition is observed between 280 and 300 K, which matches resistivity measurements. Moreover, the activation energy of the electron hopping conduction above the phase transition is predicted to be 0.18 eV deviating only 0.02 eV from experiment. This work demonstrates that machine learning is able to provide an accurate representation of both, the geometric and the electronic structure dynamics of Li$_x$Mn$_2$O$_4$, on time and length scales that are not accessible by ab initio MD.",2007.00335v2 2022-08-19,Superconductivity of Cs$_3$C$_{60}$ at atmosphere pressure,"Pressure as a clean and efficient tool can bring about unexpected extraordinary physical and chemical properties of matters. The recent discoveries of superconductivity at nearly room temperature in hydrides highlight the power of pressure in this aspect. Capturing such Tc superconductivity at atmosphere pressure for the technological applications is highly desired. The large-scale growth of diamond through the chemical vapor deposition away from the usual high-pressure and high-temperature conditions fuels such a hope. Similar to hydrides, Cs-doped C$_{60}$ was also found to exhibit superconductivity by the application of pressure with a comparable Tc of 40 K as MgB$_2$. Here, we report the successful realization of superconductivity in Cs-doped C$_{60}$ at atmosphere pressure. The phase is characterized to have the primitive cubic structure in the space group of Pa-3 with the stoichiometry of Cs$_3$C$_{60}$. The superconductivity is evidenced from the observations of both the Meissner effect and zero-resistance state. Although the pressure effects on superconductivity are different for the newly discovered Cs$_{3}$C$_{60}$ compared to the known two phases with fcc and A15 structure, the evolution of Tc with the volume for all these superconductors follows the same universal trend, suggesting the same pairing mechanism of the superconductivity. Such a trend together with the nearly linear Tc vs the lattice constant in the structure with smaller unit-cell volumes and the neighbouring antiferromagnetic state in the structure with larger unit-cell volumes invites the electron-phonon coupling and the electron correlations together to account for the superconductivity in Cs$_3$C$_{60}$. The present results and findings suggest a new route to capturing the superconductivity which takes place at high pressures to atmosphere pressure environment.",2208.09429v1 2022-11-02,High Temperature Ferromagnetism in Cr$_{1+x}$Pt$_{5-x}$P,"We present the growth and basic magnetic and transport properties of Cr$_{1+x}$Pt$_{5-x}$P. We show that single crystals can readily be grown from a high-temperature solution created by adding dilute quantities of Cr to Pt-P based melts. Like other 1-5-1 compounds, Cr$_{1+x}$Pt$_{5-x}$P adopts a tetragonal P4/mmm structure composed face-sharing CrPt$_3$ like slabs that are broken up along the c-axis by sheets of P atoms. EDS and X-ray diffraction measurements both suggest Cr$_{1+x}$Pt$_{5-x}$P has mixed occupancy between Cr and Pt atoms, similar to what is found in the closely related compound CrPt$_3$, giving real compositions of Cr$_{1.5}$Pt$_{4.5}$P (x = 0.5). We report that Cr$_{1.5}$Pt$_{4.5}$P orders ferromagnetically at T$_C$ = 464.5 K with a saturated moment of $\approx$ 2.1 $\mu_{\textit{B}}$/Cr at 1.8 K. Likely owing to the strong spin-orbit coupling associated with the large quantity of high Z Pt atoms, Cr$_{1.5}$Pt$_{4.5}$P has exceptionally strong planar anisotropy with estimated anisotropy fields of 345 kOe and 220 kOe at 1.8 K and 300 K respectively. The resistance of Cr$_{1.5}$Pt$_{4.5}$P has a metallic temperature dependence with relatively weak magnetoresistance. Electronic band structure calculations show that CrPt$_5$P has a large peak in the density of states near the Fermi level which is split into spin majority and minority bands in the ferromagnetic state. Furthermore, the calculations suggest substantial hybridization between Cr-3d and Pt-5d states near the Fermi level, in agreement with the experimentally measured anisotropy.",2211.01491v1 2020-01-22,Spintronic superconductor in a bulk layered material with natural spin-valve structure,"Multi-layered materials provide fascinating platforms to realize various functional properties, possibly leading to future electronic devices controlled by external fields. In particular, layered magnets coupled with conducting layers have been extensively studied recently for possible control of their transport properties via the spin structure. Successful control of quantum-transport properties in the materials with antiferromagnetic (AFM) layers, so-called natural spin-valve structure, has been reported for the Dirac Fermion and topological/axion materials. However, a bulk crystal in which magnetic and superconducting layers are alternately stacked has not been realized until now, and the search for functional properties in it is an interesting yet unexplored field in material science. Here, we discover superconductivity providing such an ideal platform in EuSn2As2 with the van der Waals stacking of magnetic Eu layers and superconducting Sn-As layers, and present the first demonstration of a natural spin-valve effect on the superconducting current. Below the superconducting transition temperature (Tc), the electrical resistivity becomes zero in the in-plane direction. In contrast, it, surprisingly, remains finite down to the lowest temperature in the out-of-plane direction, mostly due to the structure of intrinsic magnetic Josephson junctions in EuSn2As2. The magnetic order of the Eu layers (or natural spin-valve) is observed to be extremely soft, allowing one to easy control of the out-of-plane to in-plane resistivities ratio from 1 to infinity by weak external magnetic fields. The concept of multi-functional materials with stacked magnetic-superconducting layers will open a new pathway to develop novel spintronic devices with magnetically controllable superconductivity.",2001.07991v1 1997-02-26,"Stripes, Non-Fermi-Liquid Behavior, and High-Tc Superconductivity","The electronic structure of the high-Tc cuprates is studied in terms of ""large-U"" and ""small-U"" orbitals. A striped structure and three types of quasiparticles are obtained, polaron-like ""stripons"" carrying charge, ""svivons"" carrying spin, and ""quasielectrons"" carrying both. The anomalous properties are explained, and specifically the behavior of the resistivity, Hall constant, and thermoelectric power. High-temperature superconductivity results from transitions between pair states of quasielectrons and stripons.",9702232v1 2014-12-09,Materials Cartography: Representing and Mining Material Space Using Structural and Electronic Fingerprints,"As the proliferation of high-throughput approaches in materials science is increasing the wealth of data in the field, the gap between accumulated-information and derived-knowledge widens. We address the issue of scientific discovery in materials databases by introducing novel analytical approaches based on structural and electronic materials fingerprints. The framework is employed to (i) query large databases of materials using similarity concepts, (ii) map the connectivity of the materials space (i.e., as a materials cartogram) for rapidly identifying regions with unique organizations/properties, and (iii) develop predictive Quantitative Materials Structure-Property Relation- ships (QMSPR) models for guiding materials design. In this study, we test these fingerprints by seeking target material properties. As a quantitative example, we model the critical temperatures of known superconductors. Our novel materials fingerprinting and materials cartography approaches contribute to the emerging field of materials informatics by enabling effective computational tools to analyze, visualize, model, and design new materials.",1412.4096v3 2013-10-14,High Pressure Effects on the Superconductivity in Rare-Earth Doped CaFe2As2,"High-pressure superconductivity in a rare-earth doped Ca0.86Pr0.14Fe2As2 single crystalline sample has been studied up to 12 GPa and temperatures down to 11 K using designer diamond anvil cell under a quasi-hydrostatic pressure medium. The electrical resistance measurements were complemented by high pressure and low temperature x-ray diffraction studies at a synchrotron source. The electrical resistance measurements show an intriguing observation of superconductivity under pressure, with Tc as high as ~51 K at 1.9 GPa, presenting the highest Tc reported in the intermetallic class of 1-2-2 iron-based superconductors. The resistive transition observed suggests a possible existence of two superconducting phases at low pressures of 0.5 GPa: one phase starting at Tc1 ~48 K, and the other starting at Tc2~16 K. The two superconducting transitions show distinct variations with increasing pressure. High pressure low temperature structural studies indicate that the superconducting phase is a collapsed tetragonal ThCr2Si2-type (122) crystal structure. Our high pressure studies indicate that high Tc state attributed to non-bulk superconductivity in rare-earth doped 1-2-2 iron-based superconductors is stable under compression over a broad pressure range.",1310.3842v2 2022-04-01,Magnetic Kagome Superconductor CeRu$_2$,"Materials with a kagome lattice provide a platform for searching for new electronic phases and investigating the interplay between correlation and topology. Various probes have recently shown that the kagome lattice can host diverse quantum phases with intertwined orders, including charge density wave states, bond density wave states, chiral charge order, and, rarely, superconductivity. However, reports of the coexistence of superconductivity and magnetic order in kagome materials remain elusive. Here we revisit a magnetic superconductor CeRu$_2$ with a kagome network formed by Ru atoms. Our first-principles calculations revealed a kagome flat band near the Fermi surface, indicative of flat-band magnetism. At ambient pressure, CeRu$_2$ exhibits a superconducting transition temperature ($T_{\text{c}}$) up to ~ 6 K and a magnetic order at ~ 40 K. Notably, superconductivity and related behavior can be tuned by adjusting the amount of Ru. We conducted a systematic investigation of the superconductivity and magnetic order in CeRu$_2$ via magnetic, resistivity, and structural measurements under pressure up to ~ 168 GPa. An unusual phase diagram that suggests an intriguing interplay between the compound's superconducting order parameters has been constructed. A $T_{\text{c}}$ resurgence was observed above pressure of ~ 28 GPa, accompanied by the sudden appearance of a secondary superconducting transition. Our experiments have identified tantalizing phase transitions driven by high pressure and suggest that the superconductivity and magnetism in CeRu$_2$ are strongly intertwined.",2204.00553v2 2004-12-06,"Resistivity and Thermoelectric power of NaxCoO2 (x =1.0, 0.7 and 0.6) system","Results of thermo-electric power (S) and electrical resistivity (r) measurements are reported on NaxCoO2 compounds with x = 1.0, 0.7 and 0.6. These are single-phase compounds crystallizing in the hexagonal structure (space group P63/mmc) at room temperature. Thermo-electric power values at 300K (S300K) are, 80mV/K, 39mV/K and 37mV/K for x = 1.0, 0.7 and 0.6 samples, respectively. The samples with x=0.7 and 1.0 are metallic down to 5 K, while the x = 0.6 sample is semiconducting. The value of r300K for x = 1.0 sample is \~0.895 mW-cm and the power factor (S2/r) is = 7.04 x 10-3 W/mK2 which qualifies it as a good thermo-electric material. In x =1.0 sample, S(T) is positive throughout 300-5K temperature range and decreases monotonically to zero as temperature T= 0. In contrast, S(T) of x = 0.7 and 0.6 samples changes sign and shows negative values between 90 K and 16 K before approaching zero as T = 0. Anomalous S(T) behavior of x = 0.6 and 0.7 samples, which are coincidentally the precursor materials to the reported superconductivity in this class of materials, indicates a dramatic change in the electronic structure of these compounds on lowering the Na content.",0412122v1 2011-11-21,"Anisotropic Magnetoresistance Effects in Fe, Co, Ni, Fe_4N, and Half-Metallic Ferromagnet: A Systematic Analysis","We theoretically analyze the anisotropic magnetoresistance (AMR) effects of bcc Fe (+), fcc Co (+), fcc Ni (+), Fe$_4$N (-), and a half-metallic ferromagnet (-). The sign in each ( ) represents the sign of the AMR ratio observed experimentally. We here use the two-current model for a system consisting of a spin-polarized conduction state and localized d states with spin--orbit interaction. From the model, we first derive a general expression of the AMR ratio. The expression consists of a resistivity of the conduction state of the $\sigma$ spin ($\sigma=\uparrow$ or $\downarrow$), $\rho_{s \sigma}$, and resistivities due to s--d scattering processes from the conduction state to the localized d states. On the basis of this expression, we next find a relation between the sign of the AMR ratio and the s--d scattering process. In addition, we obtain expressions of the AMR ratios appropriate to the respective materials. Using the expressions, we evaluate their AMR ratios, where the expressions take into account the values of $\rho_{s \downarrow}/\rho_{s \uparrow}$ of the respective materials. The evaluated AMR ratios correspond well to the experimental results.",1111.4864v3 2013-09-25,Piezoresistance in Silicon and its nanostructures,"Piezoresistance is the change in the electrical resistance, or more specifically the resistivity, of a solid induced by an applied mechanical stress. The origin of this effect in bulk, crystalline materials like Silicon, is principally a change in the electronic structure which leads to a modification of the charge carriers effective mass. The last few years have seen a rising interest in the piezoresistive properties of semiconductor nanostructures, motivated in large part by claims of a giant piezoresistance effect in Silicon nanowires that is more than two orders of magnitude bigger than the known bulk effect. This review aims to present the controversy surrounding claims and counter-claims of giant piezoresistance in Silicon nanostructures by presenting a summary of the major works carried out over the last 10 years. The main conclusions that can be drawn from the literature are that i) reproducible evidence for a giant piezoresistance effect in un-gated Silicon nanowires is limited, ii) in gated nanowires a giant effect has been reproduced by several authors, iii) the giant effect is fundamentally different from either the bulk Silicon piezoresistance or that due to quantum confinement in accumulation layers and heterostructures, the evidence pointing to an electrostatic origin for the piezoresistance, iv) released nanowires tend to have slightly larger piezoresistance coefficients than un-released nanowires, and v) insufficient work has been performed on bottom-up grown nanowires to be able to rule out a fundamental difference in their properties when compared with top-down nanowires. On the basis of this, future possible research directions are suggested.",1309.6445v2 2014-09-25,Superconductivity in 122-type antimonide BaPt$_2$Sb$_2$,"The crystal structure, superconducting properties, and electronic structure of a novel superconducting 122-type antimonide, BaPt$_2$Sb$_2$, have been investigated by measurements of powder X-ray diffraction patterns, electrical resistivity, ac magnetic susceptibility, specific heat as well as ab-initio calculations. This material crystallizes in a new-type of monoclinic variant of the CaBe$_2$Ge$_2$-type structure, in which Pt$_2$Sb$_2$ layers consisting of PtSb$_4$ tetrahedra and Sb$_2$Pt$_2$ layers consisting of SbPt$_4$ tetrahedra are stacked alternatively and Ba atoms are located between the layers. Measurements of electrical resistivity, ac magnetic susceptibility and specific heat revealed that BaPt$_2$Sb$_2$ is a superconducting material with a $T_{\rm c}$ of 1.8 K. The electronic heat capacity coefficient $\gamma_{\rm n}$ and Debye temperature $\theta_{\rm D}$ were 8.6(2) mJ/mol K$^2$ and 146(4) K, where the figures in parentheses represent the standard deviation. The upper critical field $\mu_{\rm 0}H_{\rm c2}(0)$ and the Ginzburg-Landau coherent length $\xi(0)$ were determined to be 0.27 T and 35 nm. Calculations showed that it has two three-dimensional Fermi surfaces (FSs) and two two-dimensional FSs, leading to anisotropic transport properties. The d-states of the Pt atoms in the Pt2Sb2 layers mainly contribute to $N(E_{\rm F})$. A comparison between experimental and calculated results indicates that BaPt$_2$Sb$_2$ is a superconducting material with moderate coupling.",1409.7147v1 2014-11-11,Tunable Cobalt Vacancies and Related Properties in LaCoxAs2,"The origin of transition metal vacancies and their effects on the properties of ThCr2Si2-type compounds have been less studied and poorly understood. Here we carefully investigate the structure, physical properties, and electronic structure for a series of lanthanum cobalt arsenides with nominal composition of LaCoxAs2 (1.6 < = x < = 2.1). It is revealed that the occupancy of Co can be tuned between 1.98(1) and 1.61(1). The structural analyses based on X-ray and neutron diffractions show the existence of Co vacancies results from charge balance due to the formation of bond between As-As. These Co vacancies affect the magnetic and electrical properties greatly, adjusting the Curie temperature from 205 to 47 K and increasing the resistivity by more than 100%. First principles calculations indicate that the Co vacancies weaken the spin polarization and reduce the density of states at the Fermi level, resulting in decreased Curie temperature and increased resistivity, respectively. Our results address the importance of transition metal vacancies in ThCr2Si2-type materials and offer a reliable route to tune the magnetism of ThCr2Si2-type structure.",1411.2788v1 2017-10-02,Realization of the Axion Insulator State in Quantum Anomalous Hall Sandwich Heterostructures,"The 'magnetoelectric effect' arises from the coupling between magnetic and electric properties in materials. The Z2 invariant of topological insulators (TIs) leads to a quantized version of this phenomenon, known as the topological magnetoelectric (TME) effect. This effect can be realized in a new topological phase called an 'axion insulator' whose surface states are all gapped but the interior still obeys time reversal symmetry. We demonstrate such a phase using electrical transport measurements in a quantum anomalous Hall (QAH) sandwich heterostructure, in which two compositionally different magnetic TI layers are separated by an undoped TI layer. Magnetic force microscopy images of the same sample reveal sequential magnetization reversals of the top and bottom layers at different coercive fields, a consequence of the weak interlayer exchange coupling due to the spacer. When the magnetization is antiparallel, both the Hall resistance and Hall conductance show zero plateaus, accompanied by a large longitudinal resistance and vanishing longitudinal conductance, indicating the realization of an axion insulator state. Our findings thus show evidences for a phase of matter distinct from the established QAH state and provide a promising platform for the realization of the TME effect.",1710.00471v2 2018-04-20,Pressure induced superconductivity bordering a charge-density-wave state in NbTe4 with strong spinorbit coupling,"Transition-metal chalcogenides host various phases of matter, such as charge-density wave (CDW), superconductors, and topological insulators or semimetals. Superconductivity and its competition with CDW in low-dimensional compounds have attracted much interest and stimulated considerable research. Here we report pressure induced superconductivity in a strong spin-orbit (SO) coupled quasi-one-dimensional (1D) transition-metal chalcogenide NbTe$_4$, which is a CDW material under ambient pressure. With increasing pressure, the CDW transition temperature is gradually suppressed, and superconducting transition, which is fingerprinted by a steep resistivity drop, emerges at pressures above 12.4 GPa. Under pressure $p$ = 69 GPa, zero resistance is detected with a transition temperature $T_c$ = 2.2 K and an upper critical field $H_{c2}$= 2 T. We also find large magnetoresistance (MR) up to 102\% at low temperatures, which is a distinct feature differentiating NbTe$_4$ from other conventional CDW materials.",1804.07448v1 2018-11-12,Laser writable high-K dielectric for van der Waals nano-electronics,"Like silicon-based semiconductor devices, van der Waals heterostructures will require integration with high-K oxides. This is needed to achieve suitable voltage scaling, improved performance as well as allowing for added functionalities. Unfortunately, commonly used high-k oxide deposition methods are not directly compatible with 2D materials. Here we demonstrate a method to embed a multi-functional few nm thick high-k oxide within van der Waals devices without degrading the properties of the neighbouring 2D materials. This is achieved by in-situ laser oxidation of embedded few layer HfS2 crystals. The resultant oxide is found to be in the amorphous phase with a dielectric constant of k~15 and break-down electric fields in the range of 0.5-0.6 V/nm. This transformation allows for the creation of a variety of fundamental nano-electronic and opto-electronic devices including, flexible Schottky barrier field effect transistors, dual gated graphene transistors as well as vertical light emitting and detecting tunnelling transistors. Furthermore, upon dielectric break-down, electrically conductive filaments are formed. This filamentation process can be used to electrically contact encapsulated conductive materials. Careful control of the filamentation process also allows for reversible switching between two resistance states. This allows for the creation of resistive switching random access memories (ReRAMs). We believe that this method of embedding a high-k oxide within complex van der Waals heterostructures could play an important role in future flexible multi-functional van der Waals devices.",1811.04829v1 2018-10-09,"Magnetic behavior, Griffiths phase and magneto-transport study in 3$d$ based nano-crystalline double perovskite Pr$_2$CoMnO$_6$","Double perovskite (DP) oxide material receive extensive research interest due to exciting physical properties with potential technological application. 3$d$ based DP oxides are promising for exciting physics like magnetodielectric, ferroelectric, Griffith phase etc., specially Co/Mn DPs are gaining much research interest. In this paper we present the study of magnetic phase and transport properties in nano-crystalline Pr$_2$CoMnO$_6$ a 3$d$ based double perovskite compound. This material shows a paramagnetic (PM) to ferromagnetic (FM) phase transition below 173 K marked by a rapid increase in magnetic moment due to spin ordering. We found divergence in inverse magnetic susceptibility ($\chi$$^{-1}$) from Curie weiss behavior around 206 K which indicates the evolution of Griffiths phase before actual PM-FM transition. We found that the Griffiths phase suppressed with increasing applied magnetic filed. For the understanding of charge transport in this material we have measured temperature dependent electrical resistivity. Pr$_2$CoMnO$_6$ is a strong insulator where resistivity increase abruptly below magnetic phase transition. To understand the effect of magnetic field on transport behavior we have also measured the magnetoresistance (MR) at different temperatures. Sample shows the negative MR with maximum value $\sim$22 $\%$ under applied magnetic field of 50 kOe at 125 K. MR follows quadratic field dependency above $T_c$ however below $T_c$ the MR shows deviation from this field dependency at low field.",1810.03895v1 2020-02-11,A Multiscale Constitutive Model for Metal Forming of Dual Phase Titanium Alloys by Incorporating Inherent Deformation and Failure Mechanisms,"Ductile metals undergo a considerable amount of plastic deformation before failure. Void nucleation, growth and coalescence is the mechanism of failure in such metals. {\alpha}/{\beta} titanium alloys are ductile in nature and are widely used for their unique set of properties like specific strength, fracture toughness, corrosion resistance and resistance to fatigue failures. Voids in these alloys were reported to nucleate on the phase boundaries between {\alpha} and {\beta} phase. Based on the findings of crystal plasticity finite element method (CPFEM) based investigation of the void growth at the interface of {\alpha} and {\beta} phases [1], [2], a void nucleation, growth, and coalescence model has been formulated. An existing single-phase crystal plasticity theory is extended to incorporate underlying physical mechanisms of deformation and failure in dual phase titanium alloys. Effects of various factors (stress triaxiality, Lode parameter, deformation state (equivalent strain), and phase boundary inclination) on void nucleation, growth and coalescence are used to formulate the constitutive model while their interaction with a conventional crystal plasticity theory is established. An extensive parametric assessment of the model is carried out to quantify and understand the effects of the material parameters on the overall material response. Performance of the proposed model is then assessed and verified by comparing the results of the proposed model with the RVE study results. Application of the constitutive model for utilisation in the design and optimisation of the forming process of {\alpha}/{\beta} titanium alloy components is also demonstrated using experimental data.",2002.04459v1 2020-04-23,Hybrid Graphene/Carbon Nanofiber Wax Emulsion for Paper-based Electronics and Thermal Management,"Materials for electronics that function as electrical and/or thermal conductors are often rigid, expensive, difficult to be sourced and sometimes toxic. An electrically and thermally conductive nanocomposite that is lightweight, flexible and eco-friendly could improve the environmental friendliness of the electronics sector and enable new applications. Considering this, we have fabricated electrically and thermally conductive flexible materials by functionalizing paper with nanocarbon conductive inks. Carnauba wax is emulsified in isopropyl alcohol and mixed with graphene nanoplatelets (GNPs) or with hybrids of GNPs and carbon nanofibers (CNFs). The percolation threshold of the hybrid samples is lowered compared with the pure GNPs composites, due to their increased filler aspect ratio. The hybrid samples also exhibit superior bending and folding stability. Densification of the coating to decrease their sheet resistance enables them to achieve as low as ~ 50 {\Omega} sq-1 for the GNP-based paper. The densification procedure improves the bending stability, the abrasion resistance, and the electromagnetic interference shielding of the paper-based conductors. Finally, the compressed samples show an impressive enhancement of their thermal diffusivity. The flexible and multifunctional nanocarbon coated paper is a promising electronic conductor and thermally dissipative material and, at the same time, can increase the environmental sustainability of the electronics sector.",2004.11476v1 2020-09-21,Photocurrent Imaging of Multi-Memristive Charge Density Wave Switching in Two-Dimensional 1T-TaS2,"Transport studies of atomically thin 1T-TaS2 have demonstrated the presence of intermediate resistance states across the nearly commensurate (NC) to commensurate (C) charge density wave (CDW) transition, which can be further switched electrically. While this presents exciting opportunities for the material in memristor applications, the switching mechanism has remained elusive and could be potentially attributed to the formation of inhomogeneous C and NC domains across the 1T-TaS2 flake. Here, we present simultaneous electrical driving and scanning photocurrent imaging of CDWs in ultrathin 1T-TaS2 using a vertical heterostructure geometry. While micron-sized CDW domains form upon changing temperature, electrically driven transitions result in largely uniform changes, indicating that states of intermediate resistance for the latter likely correspond to true metastable CDW states in between the NC and C phases, which we then explain by a free energy analysis. Additionally, we are able to perform repeatable and bidirectional switching across the multiple CDW states without changing sample temperature, demonstrating that atomically thin 1T-TaS2 can be further used as a robust and reversible multi-memristor material.",2009.10179v1 2018-12-21,Transfer of mass and momentum at rough and porous surfaces,"The surface texture of materials plays a critical role in wettability, turbulence and transport phenomena. In order to design surfaces for these applications, it is desirable to characterise non-smooth and porous materials by their ability to exchange mass and momentum with flowing fluids. While the underlying physics of the tangential (slip) velocity at a fluid-solid interface is well understood, the importance and treatment of normal (transpiration) velocity and normal stress is unclear. We show that, when slip velocity varies at an interface above the texture, a non-zero transpiration velocity arises from mass conservation. The ability of a given surface texture to accommodate for a normal velocity of this kind is quantified by a transpiration length. We further demonstrate that normal momentum transfer gives rise to a pressure jump. For a porous material, the pressure jump can be characterised by so called resistance coefficients. By solving five Stokes problems, the introduced measures of slip, transpiration and resistance can be determined for any anisotropic non-smooth surface consisting of regularly repeating geometric patterns. The proposed conditions are a subset of effective boundary conditions derived from formal multi-scale expansion. We validate and demonstrate the physical significance of the effective conditions on two canonical problems -- a lid-driven cavity and a turbulent channel flow, both with non-smooth bottom surfaces.",1812.09401v2 2019-06-25,Titanium Contacts to MoS2 with Interfacial Oxide: Interface Chemistry and Thermal Transport,"The deposition of a thin oxide layer at metal/semiconductor interfaces has been previously reported as a means of reducing contact resistance in 2D electronics. Using X-ray photoelectron spectroscopy with in-situ Ti deposition, we fabricate Au/Ti/TiOx/MoS2 samples as well as Au/Ti/MoS2 and Au/TiOx/MoS2 for comparison. Elemental titanium reacts strongly with MoS2 whereas no interface reactions are observed in the two types of samples containing TiOx/MoS2 interfaces. Using time domain thermoreflectance for the measurement of thermal boundary conductance, we find that samples contacted with Ti and a thin TiOx layer at the interface (less than or equal to 1.5 nm) exhibit the same behavior as samples contacted solely with pure Ti. The Au/TiOx/MoS2 samples exhibit approximately 20% lower thermal boundary conductance, despite having the same MoS2 interface chemistry as the samples with thin oxide at the Ti/MoS2 interface. We identify the mechanism for this phenomenon, attributing it to the different interfaces with the top Au contact. Our work demonstrates that the use of thin interfacial oxide layers to reduce electrical contact resistance does not compromise heat flow in 2D electronic devices. We note that the thicknesses of the Ti and TiOx layers must be considered for optimal thermal transport.",1906.10727v1 2019-06-27,The Essential Work of Fracture Parameters for 3D printed polymer sheets,"Additive manufacturing is becoming increasingly popular in academia and industry. Accordingly, there has been a growing interest in characterizing 3D printed samples to determine their structural integrity behaviour. We employ the Essential Work of Fracture (EWF) to investigate the mechanical response of polymer sheets obtained through additive manufacturing. Our goal is twofold; first, we aim at gaining insight into the role of fibre reinforcement on the fracture resistance of additively manufactured polymer sheets. Deeply double-edge notched tensile (DDEN-T) tests are conducted on four different polymers: Onyx, a crystalline, nylon-reinforced polymer, and three standard polymers used in additive manufacturing - PLA, PP and ABS. Results show that fibre-reinforcement translates into a notable increase in fracture resistance, with the fracture energy of Onyx being an order of magnitude higher than that reported for non-reinforced polymers. On the other hand, we propose the use of a miniature test specimen, the deeply double-edge notched small punch specimens (DDEN-SP), to characterize the mechanical response using a limited amount of material. The results obtained exhibit good alignment with the DDEN-T data, suggesting the suitability of the DDEN-SP test for measuring fracture properties of additively manufactured polymers in a cost-effective manner.",1906.11512v1 2019-10-09,"The roles of adhesion, internal heat generation and elevated temperatures in normally loaded, sliding rough surfaces","The thermal effects of plastic and frictional heat generation and elevated temperature were examined along with the role of adhesion in the context of galling wear, using a representative crystal plasticity, normally loaded, sliding surface model. Galling frequency behaviour was predicted for 316L steel. Deformation of the surfaces was dominated by the surface geometry, with no significant effect due to variations in frictional models. Plastic and frictional heating were found to have a minimal effect on the deformation of the surface, with the rapid conduction of heat preventing any highly localised heating. There was no corresponding effect on the predicted galling frequency response. Isothermal, elevated temperature conditions caused a decrease in galling resistance, driven by the temperature sensitivity of the critical resolved shear stress. The extent of deformation, as quantified by the area of plastically deformed material and plastic reach, increased with temperature. Comparisons were made with literature results for several surface amplitude and wavelength conditions. Model results compared favourably with those in the literature. However, the reduction in predicted galling resistance with elevated temperature for a fixed surface was not as severe as observations in the literature, suggesting other mechanisms (e.g. phase transformations, surface coatings and oxides) are likely important.",1910.03830v1 2020-01-06,Two-dimensional antiferroelectric tunnel junction,"Ferroelectric tunnel junctions (FTJs), which consist of two metal electrodes separated by a thin ferroelectric barrier, have recently aroused significant interest for technological applications as nanoscale resistive switching devices. So far, most of existing FTJs have been based on perovskite-oxide barrier layers. The recent discovery of the two-dimensional (2D) van der Waals ferroelectric materials opens a new route to realize tunnel junctions with new functionalities and nm-scale dimensions. Due to the weak coupling between the atomic layers in these materials, the relative dipole alignment between them can be controlled by applied voltage. This allows transitions between ferroelectric and antiferroelectric orderings, resulting in significant changes of the electronic structure. Here, we propose to realize 2D antiferroelectric tunnel junctions (AFTJs), which exploit this new functionality, based on bilayer In$_2$X$_3$ (X = S, Se, Te) barriers and different 2D electrodes. Using first-principles density functional theory calculations, we demonstrate that the In$_2$X$_3$ bilayers exhibit stable ferroelectric and antiferroelectric states separated by sizable energy barriers, thus supporting a non-volatile switching between these states. Using quantum-mechanical modeling of the electronic transport, we explore in-plane and out-of-plane tunneling across the In$_2$S$_3$ van der Waals bilayers, and predict giant tunneling electroresistance (TER) effects and multiple non-volatile resistance states driven by ferroelectric-antiferroelectric order transitions. Our proposal opens a new route to realize nanoscale memory devices with ultrahigh storage density using 2D AFTJs.",2001.01639v3 2020-01-28,Interlayer band-to-band tunneling and negative differential resistance in van der Waals BP/InSe field effect transistors,"Atomically thin layers of van der Waals (vdW) crystals offer an ideal material platform to realize tunnel field effect transistors (TFETs) that exploit the tunneling of charge carriers across the forbidden gap of a vdW heterojunction. This type of device requires a precise energy band alignment of the different layers of the junction to optimize the tunnel current. Amongst two-dimensional (2D) vdW materials, black phosphorus (BP) and indium selenide (InSe) have a Brillouin zone-centered conduction and valence bands, and a type II band offset, both ideally suited for band-to-band tunneling. Here, we demonstrate TFETs based on BP/InSe heterojunctions with diverse electrical transport characteristics: forward rectifying, Zener-tunneling and backward rectifying characteristics are realized in BP/InSe junctions with different thickness of the BP layer or by electrostatic gating of the junction. Electrostatic gating yields a large on/off current ratio of up to 108 and negative differential resistance at low applied voltages (V ~ 0.2V). These findings illustrate versatile functionalities of TFETs based on BP and InSe, offering opportunities for applications of these 2D materials beyond the device architectures reported in the current literature.",2001.10273v1 2020-08-31,Creep deformation of WC hardmetals with iron-based binders,"Iron is a candidate to replace cobalt in WC hardmetals, due to its lower cost and toxicity. A WC-FeCr hardmetal was compression tested at 900-1200 {\deg}C. Particular attention is paid to the steady-state creep rates and stress-exponents (n) during isostress treatments. Three regimes of stress dependence are observed. Two of these were previously reported for WC-Co: power law creep (n~3) at medium stresses; and grain boundary sliding (n~1) at higher stresses, generally >100MPa. A previously unreported low stress (<10MPa) regime with an exponent of n~2 is also observed. By combining electron microscopy with X-ray diffraction texture measurements, the low stress regime is attributed to viscous flow of the binder, which is accommodated by diffusional creep in the WC skeleton. The mechanism may be applicable to other hardmetals. Compared to analogous WC-Co materials, WC-FeCr shows improved creep resistance below 1000 {\deg}C, which can be explained by its lower self-diffusivity, and a lower solubility for WC than Co. However, at temperatures corresponding to liquid eutectic formation (~1140 {\deg}C), its creep resistance becomes inferior. These results indicate FeCr may be a suitable replacement for Co provided the eutectic temperature is not exceeded.",2008.13565v1 2020-10-06,Role of f-d exchange interaction and Kondo scattering in Nd doped pyrochlore Iridate (Eu1-xNdx)2Ir2O7,"We report study of magnetization, resistivity, magnetoresistance and specific heat of the pyrochlore Iridate (Eu1-xNdx)2Ir2O7 with x=0.0, 0.5 and 1.0, where spin orbit coupling, electronic correlation, magnetic frustration and Kondo scattering coexists. Metal insulator transition temperature (T_MI) decrease with increase in Nd content but always coincides with magnetic irreversibility temperature (field induced moment). Resistivity below T_MI do not fit with either activated (gap) or to any power law (gapless) dependence. The Curie constant show surprising result, that Nd induces singlet correlation (reduction of para-moment) in Ir sublattice. Magnetoresistance is negative at low temperatures below 10 K and increases strongly with increase in x and vary quadratically with field switching over to linear dependence above 50 kOe. Low temperature specific heat shows Schottky peak, coming from Nd moments, showing existence of doublet split in Nd energy level, arising from f-d exchange interaction. All materials show presence of a linear specific heat in the insulating region. The coefficient of linear specific heat for x= 0.0 does not vary with external magnetic field but varies superlinearly for x = 1.0 materials. We argue that linear specific heat probably rules out weakly correlated phases like Weyl fermions. We propose that with the introduction of Nd at Eu site the system evolves from chiral spin liquid with gapless spinon excitations with a very small charge gap to Kondo type interaction superposed on chiral spin liquid coexisting with long range antiferromagnetic ordering. Huge increase of magnetoresistance with increase in Nd concentrations shows importance of Kondo scattering in the chiral spin liquid material by rare earth moments.",2010.02685v1 2020-10-15,Multipurpose and Reusable Ultrathin Electronic Tattoos Based on PtSe2 and PtTe2,"Wearable bioelectronics with emphasis on the research and development of advanced person-oriented biomedical devices have attracted immense interest in the last decade. Scientists and clinicians find it essential to utilize skin-worn smart tattoos for on-demand and ambulatory monitoring of an individual's vital signs. Here we report on the development of novel ultrathin platinum-based two-dimensional dichalcogenide (Pt-TMDs) based electronic tattoos as advanced building blocks of future wearable bioelectronics. We made these ultrathin electronic tattoos out of large-scale synthesized platinum diselenide (PtSe2) and platinum ditelluride (PtTe2) layered materials and used them for monitoring human physiological vital signs, such as the electrical activity of the heart and the brain, muscle contractions, eye movements, and temperature. We show that both materials can be used for these applications; yet, PtTe2 was found to be the most suitable choice due to its metallic structure. In terms of sheet resistance, skin-contact, and electrochemical impedance, PtTe2 outperforms state-of-the-art gold and graphene electronic tattoos and performs on par with medical-grade Ag/AgCl gel electrodes. The PtTe2 tattoos show four times lower impedance and almost 100 times lower sheet resistance compared to monolayer graphene tattoos. One of the possible prompt implications of the work is perhaps in the development of advanced human-machine interfaces. To display the application, we built a multi-tattoo system that can easily distinguish eye movement and identify the direction of an individual's sight.",2010.07534v1 2020-10-22,"Development, Processing and Applications of a UV-Curable Polymer with Surface Active Thiol Groups","We present here a novel resist formulation with active thiol groups at the surface. The material is UV curable, and can be patterned at the micro- and nanoscale by UV nanoimprint lithography. The resist formulation development, its processing, patterning and surface characterization are presented here. In addition, a possible application, including its use to modify the electrical properties of graphene devices is shown. The cured material is highly transparent, intrinsically hydrophilic and can be made more hydrophilic following a UV-ozone or an O2 plasma activation. We evaluated the hydrophilicity of the polymer for different polymer formulations and curing conditions. In addition, a protocol for patterning of the polymer in the micro and nanoscale by nanoimprinting is given and preliminary etching rates together with the polymer selectivity are measured. The main characteristic and unique advantage of the polymer is that it has thiol functional groups at the surface and in the bulk after curing. These groups allow for direct surface modifications with thiol-based chemistry e.g., thiol-ene reactions. We prove the presence of the thiol groups by Raman spectroscopy and perform a thiol-ene reaction to show the potential of the easy click chemistry. This opens the way for very straightforward surface chemistry on nanoimprinted polymer samples. Furthermore, we show how the polymer improves the electrical properties of a graphene field effect transistor, allowing for optimal performance at ambient conditions.",2010.11878v1 2021-04-02,"Crystal, local atomic and electronic structures of YbFe$_2$Zn$_{20-x}$Cd$_x$ ($0 \leq x \leq 1.4$): a multi-band system with possible coexistence of light and heavy fermions","The partial (up to 7 %) substitution of Cd for Zn in the Yb-based heavy-fermion material YbFe$_2$Zn$_{20}$ is known to induce a slight ($\sim 20$ %) reduction of the Sommerfeld specific heat coefficient $\gamma$ and a huge (up to two orders of magnitude) reduction of the $T^2$ resistivity coefficient $A$, corresponding to a drastic and unexpected reduction of the Kadowaki-Woods ratio $A/\gamma ^2$. Here, Yb $L_{3}$-edge X-ray absorption spectroscopy shows that the Yb valence state is close to $3+$ for all $x$, whereas X-ray diffraction reveals that Cd replace the Zn ions only at the $16c$ site of the $Fd\bar{3}m$ cubic structure, leaving the $48f$ and $96g$ sites with full Zn occupation. Ab-initio electronic structure calculations in pure and Cd-doped materials, carried out without considering correlations, show multiple conduction bands with only minor modifications of the band dispersions near the Fermi level and therefore do not explain the resistivity drop introduced by Cd substitution. We propose that the site-selective Cd substitution introduces light conduction bands with substantial contribution of Cd($16c$) $5p$ levels that have weak coupling to the Yb$^{3+}$ $4f$ moments. These light fermions coexist with heavy fermions originated from other conduction bands with larger participation of Zn($48f$ and $96g$) $4p$ levels that remain strongly coupled with the Yb$^{3+}$ local moments.",2104.01050v1 2021-08-18,Robust narrow-gap semiconducting behavior in square-net La$_{3}$Cd$_{2}$As$_{6}$,"ABSTRACT: Narrow-gap semiconductors are sought-after materials due to their potential for long-wavelength detectors, thermoelectrics, and more recently non-trivial topology. Here we report the synthesis and characterization of a new family of narrow-gap semiconductors, $R$$_{3}$Cd$_{2}$As$_{6}$ ($R=$ La, Ce). Single crystal x-ray diffraction at room temperature reveals that the As square nets distort and Cd vacancies order in a monoclinic superstructure. A putative charge-density ordered state sets in at 279~K in La$_{3}$Cd$_{2}$As$_{6}$ and at 136~K in Ce$_{3}$Cd$_{2}$As$_{6}$ and is accompanied by a substantial increase in the electrical resistivity in both compounds. The resistivity of the La member increases by thirteen orders of magnitude on cooling, which points to a remarkably clean semiconducting ground state. Our results suggest that light square net materials within a $I4/mmm$ parent structure are promising clean narrow-gap semiconductors.",2108.08006v1 2021-10-01,"Effects of nonmagnetic impurities and subgap states on the kinetic inductance, complex conductivity, quality factor and depairing current density","We investigate how a combination of a nonmagnetic-impurity scattering rate $\gamma$ and finite subgap states parametrized by Dynes $\Gamma$ affects various physical quantities relevant to to superconducting devices: kinetic inductance $L_k$, complex conductivity $\sigma$, surface resistance $R_s$, quality factor $Q$, and depairing current density $J_d$. All the calculations are based on the Eilenberger formalism of the BCS theory. We assume the device materials are extreme type-II $s$-wave superconductors. It is well known that the optimum impurity concentration ($\gamma/\Delta_0 \sim 1$) minimizes $R_s$. Here, $\Delta_0$ is the pair potential for the idealized ($\Gamma\to 0$) superconductor for the temperature $T\to 0$. We find the optimum $\Gamma$ can also reduce $R_s$ by one order of magnitude for a clean superconductor ($\gamma/\Delta_0 < 1$) and a few tens $\%$ for a dirty superconductor ($\gamma/\Delta_0 > 1$). Also, we find a nearly-ideal ($\Gamma/\Delta_0 \ll 1$) clean-limit superconductor exhibits a frequency-independent $R_s$ for a broad range of frequency $\omega$, which can significantly improve $Q$ of a very compact cavity with a few tens of GHz frequency. As $\Gamma$ or $\gamma$ increases, the plateau disappears, and $R_s$ obeys the $\omega^2$ dependence. The subgap-state-induced residual surface resistance $R_{\rm res}$ is also studied, which can be detected by an SRF-grade high-$Q$ 3D resonator. We calculate $L_k(\gamma, \Gamma,T)$ and $J_d(\gamma, \Gamma,T)$, which are monotonic increasing and decreasing functions of $(\gamma, \Gamma,T)$, respectively. Measurements of $(\gamma, \Gamma)$ of device materials can give helpful information on engineering $(\gamma, \Gamma)$ via materials processing, by which it would be possible to improve $Q$, engineer $L_k$, and ameliorate $J_d$.",2110.00573v1 2021-10-21,Angular harmonic Hall voltage and magnetoresistance measurements of Pt/FeCoB and Pt-Ti/FeCoB bilayers for spin Hall conductivity determination,"Materials with significant spin-orbit coupling enable efficient spin-to-charge interconversion, which can be utilized in novel spin electronic devices. A number of elements, mainly heavy-metals (HM) have been identified to produce a sizable spin current ($j_\mathrm{s}$), while supplied with a charge current ($j$), detected mainly in the neighbouring ferromagnetic (FM) layer. Apart from the spin Hall angle $\theta_\mathrm{SH}$ = $j_\mathrm{s}$/$j$, spin Hall conductivity ($\sigma_\mathrm{SH}$) is an important parameter, which takes also the resistivity of the material into account. In this work, we present a measurement protocol of the HM/FM bilayers, which enables for a precise $\sigma_\mathrm{SH}$ determination. Static transport measurements, including resistivity and magnetization measurements are accompanied by the angular harmonic Hall voltage analysis in a dedicated low-noise rotating probe station. Dynamic characterization includes effective magnetization and magnetization damping measurement, which enable HM/FM interface absorption calculation. We validate the measurement protocol in Pt and Pt-Ti underlayers in contact with FeCoB and present the $\sigma_\mathrm{SH}$ of up to 3.3$\times$10$^5$ S/m, which exceeds the values typically measured in other HM, such as W or Ta.",2110.11483v1 2021-12-23,Hydrogen induced electronic transition within correlated perovskite nickelates with heavy rare-earth composition,"Although discovery in hydrogen induced electronic transition within perovskite family of rare-earth nickelate (ReNiO3) opens up a new paradigm in exploring both the new materials functionality and device applications, the existing research stays at ReNiO3 with light rare-earth compositions. To further extend the cognition towards heavier rare-earth, herein we demonstrate the hydrogen induced electronic transitions for quasi-single crystalline ReNiO3/LaAlO3 (001) heterostructures, covering a large variety of the rare-earth composition from Nd to Er. The hydrogen induced elevations in the resistivity of ReNiO3 (RH/R0) show an unexpected non-monotonic tendency with the atomic number of the rare-earth composition, e.g., firstly increase from Nd to Dy and afterwards decreases from Dy to Er. Although ReNiO3 with heavy rare-earth composition (e.g. DyNiO3) exhibits large RH/R0 up to 107, their hydrogen induced electronic transition is not reversible. Further probing the electronic structures via near edge X-ray absorption fine structure analysis clearly demonstrates the respective transition in electronic structures of ReNiO3 from Ni3+ based electron itinerant orbital configurations towards the Ni2+ based electron localized state. Balancing the hydrogen induced transition reversibility with the abruption in the variations of material resistivity, we emphasize that the ReNiO3 with middle rare-earth compositions (e.g. Sm) to be most suitable that caters for the potential applications in correlated electronic devices.",2112.12357v1 2022-12-01,Extrinsic to intrinsic mechanism crossover of anomalous Hall effect in the Ir-doped MnPtSn Heusler system,"Recent findings of large anomalous Hall signal in nonferromagnetic and nonferrimagnetic materials suggest that the magnetization of the system is not a critical component for the realization of the anomalous Hall effect (AHE). Here, we present a combined theoretical and experimental study demonstrating the evolution of different mechanisms of AHE in a cubic Heusler system MnPt$_{1-x}$Ir$_x$Sn. With the help of magnetization and neutron diffraction studies, we show that the substitution of nonmagnetic Ir in place of Pt significantly reduces the net magnetic moment from 4.17 $ \mu _B$/f.u. in MnPtSn to 2.78 $ \mu _B$/f.u. for MnPt$_{0.5}$Ir$_{0.5}$Sn. In contrast, the anomalous Hall resistivity is enhanced by nearly three times from 1.6 $ \mu \Omega $ cm in MnPtSn to about 5 $ \mu \Omega $ cm for MnPt$_{0.5}$Ir$_{0.5}$Sn. The power law analysis of the Hall resistivity data suggests that the extrinsic contribution of AHE that dominates in the case of the parent MnPtSn almost vanishes for MnPt$_{0.5}$Ir$_{0.5}$Sn, where the intrinsic mechanism plays the major role. The experimental results are well supported by our theoretical study, which shows a considerable enhancement of the spin-orbit coupling when Ir is introduced into the system. Our finding of a crossover of the anomalous Hall effect with chemical engineering is a major contribution toward the recent interest in controlling the band topology of topological materials, both in bulk and thin-film forms.",2212.00360v1 2023-06-26,Large electro-opto-mechanical coupling in VO2 neuristors,"Biological neurons are electro-mechanical systems, where the generation and propagation of an action potential is coupled to generation and transmission of an acoustic wave. Neuristors, such as VO2, characterized by insulator-metal transition (IMT) and negative differential resistance, can be engineered as self-oscillators, which are good approximations of biological neurons in the domain of electrical signals. In this study, we show that these self-oscillators are coupled electro-opto-mechanical systems, with better energy conversion coefficients than the conventional electromechanical or electrooptical materials. This is due to the significant contrast in the material's resistance, optical refractive index and density across the induced temperature range in a Joule heating driven IMT. We carried out laser interferometry to measure the opto-mechanical response while simultaneously driving the devices electrically into self-oscillations of different kinds. We analyzed films of various thicknesses, engineered device geometry and performed analytical modelling to decouple the effects of refractive index change vis-a-vis mechanical strain in the interferometry signal. We show that the effective piezoelectric coefficient (d13*) for our neuristor devices is 660 pm/V, making them viable alternatives to Pb-based piezoelectrics for MEMS applications. Furthermore, we show that the effective electro-optic coefficient (r13*) is ~22 nm/V, which is much larger than that in thin-film and bulk Pockels materials.",2306.14367v1 2023-08-28,Crystal-Chemical Origins of the Ultrahigh Conductivity of Metallic Delafossites,"Despite their highly anisotropic complex-oxidic nature, certain delafossite compounds (e.g., PdCoO2, PtCoO2) are the most conductive oxides known, for reasons that remain poorly understood. Their room-temperature conductivity can exceed that of Au, while their low-temperature electronic mean-free-paths reach an astonishing 20 microns. It is widely accepted that these materials must be ultrapure to achieve this, although the methods for their growth (which produce only small crystals) are not typically capable of such. Here, we first report a new approach to PdCoO2 crystal growth, using chemical vapor transport methods to achieve order-of-magnitude gains in size, the highest structural qualities yet reported, and record residual resistivity ratios (>440). Nevertheless, the first detailed mass spectrometry measurements on these materials reveal that they are not ultrapure, typically harboring 100s-of-parts-per-million impurity levels. Through quantitative crystal-chemical analyses, we resolve this apparent dichotomy, showing that the vast majority of impurities are forced to reside in the Co-O octahedral layers, leaving the conductive Pd sheets highly pure (~1 ppm impurity concentrations). These purities are shown to be in quantitative agreement with measured residual resistivities. We thus conclude that a previously unconsidered ""sublattice purification"" mechanism is essential to the ultrahigh low-temperature conductivity and mean-free-path of metallic delafossites.",2308.14257v2 2023-10-26,Slow and Non-Equilibrium Dynamics due to Electronic Ferroelectricity in a Strongly-Correlated Molecular Conductor,"Using a combination of resistance fluctuation (noise) and dielectric spectroscopy we investigate the nature of relaxor-type electronic ferroelectricity in the organic conductor $\kappa$-(BETS)$_2$Mn[N(CN)$_2$]$_3$, a system representative for a wider class of materials, where strong correlations of electrons on a lattice of dimerized molecules results in an insulating ground state. The two complementary spectroscopies reveal a distinct low-frequency dynamics. By dielectric spectroscopy we detect an intrinsic relaxation that is typical for relaxor ferroelectrics below the metal-to-insulator transition at $T_{\rm{MI}}\sim 25\,$K. Resistance noise spectroscopy reveals fluctuating two-level processes above $T_{\rm MI}$ which strongly couple to the applied electric field, a signature of fluctuating polar nanoregions (PNR), i.e. clusters of quantum electric dipoles fluctuating collectively. The PNR preform above the metal insulator transition. Upon cooling through $T_{\rm MI}$, a drastic increase of the low-frequency $1/f$-type fluctuations and slowing down of the charge carrier dynamics is accompanied by the onset of strong non-equilibrium dynamics indicating a glassy transition of interacting dipolar clusters, the scaling properties of which are consistent with a droplet model. The freezing of nano-scale polar clusters and non-equilibrium dynamics is suggested to be a common feature of organic relaxor-type electronic ferroelectrics and needs to be considered in theoretical models describing these materials.",2310.17242v2 2024-01-01,Nonlinear charge transport induced by gate voltage oscillation in few-layer MnBi2Te4,"Nonlinear charge transport, including nonreciprocal longitudinal resistance and nonlinear Hall effect, has garnered significant attention due to its ability to explore inherent symmetries and topological properties of novel materials. An exciting recent progress along this direction is the discovery of significant nonreciprocal longitudinal resistance and nonlinear Hall effect in the intrinsic magnetic topological insulator MnBi2Te4 induced by the quantum metric dipole. Given the importance of this finding, the inconsistent response with charge density, and conflicting requirement of C3z symmetry, it is imperative to elucidate every detail that may impact the nonlinear transport measurement. In this study, we reveal an intriguing experimental factor that inevitably gives rise to sizable nonlinear transport signal in MnBi2Te4. We demonstrate that this effect stems from the gate voltage oscillation caused by the application of a large alternating current to the sample. Furthermore, we propose a methodology to significantly suppress this effect by individually grounding the voltage electrodes during the second-harmonic measurements. Our investigation emphasizes the critical importance of thoroughly assessing the impact of gate voltage oscillation before determining the intrinsic nature of nonlinear transport in all 2D material devices with an electrically connected operative gate electrode.",2401.00679v1 1997-12-15,Spin Tunneling in Conducting Oxides,"Direct tunneling in ferromagnetic junctions is compared with impurity-assisted, surface state assisted, and inelastic contributions to a tunneling magnetoresistance (TMR). Theoretically calculated direct tunneling in iron group systems leads to about a 30% change in resistance, which is close to experimentally observed values. It is shown that the larger observed values of the TMR might be a result of tunneling involving surface polarized states. We find that tunneling via resonant defect states in the barrier radically decreases the TMR (down to 4% with Fe-based electrodes), and a resonant tunnel diode structure would give a TMR of about 8%. With regards to inelastic tunneling, magnons and phonons exhibit opposite effects: one-magnon emission generally results in spin mixing and, consequently, reduces the TMR, whereas phonons are shown to enhance the TMR. The inclusion of both magnons and phonons reasonably explains an unusual bias dependence of the TMR. The model presented here is applied qualitatively to half-metallics with 100% spin polarization, where one-magnon processes are suppressed and the change in resistance in the absence of spin-mixing on impurities may be arbitrarily large. Even in the case of imperfect magnetic configurations, the resistance change can be a few 1000 percent. Examples of half-metallic systems are CrO$_2$/TiO$_2$ and CrO$_2$/RuO$_2$, and an account of their peculiar band structures is presented. The implications and relation of these systems to CMR materials which are nearly half-metallic, are discussed.",9712170v2 2000-09-14,Experimental study of negative photoconductivity in n-PbTe(Ga) epitaxial films,"We report on low-temperature photoconductivity (PC) in n-PbTe(Ga) epitaxial films prepared by the hot-wall technique on <111>-BaF_2 substrates. Variation of the substrate temperature allowed us to change the resistivity of the films from 10^8 down to 10_{-2} Ohm x cm at 4.2 K. The resistivity reduction is associated with a slight excess of Ga concentration, disturbing the Fermi level pinning within the energy gap of n-PbTe(Ga). PC has been measured under continuous and pulse illumination in the temperature range 4.2-300 K. For films of low resistivity, the photoresponse is composed of negative and positive parts. Recombination processes for both effects are characterized by nonexponential kinetics depending on the illumination pulse duration and intensity. Analysis of the PC transient proves that the negative photoconductivity cannot be explained in terms of nonequilibrium charge carriers spatial separation of due to band modulation. Experimental results are interpreted assuming the mixed valence of Ga in lead telluride and the formation of centers with a negative correlation energy. Specifics of the PC process is determined by the energy levels attributed to donor Ga III, acceptor Ga I, and neutral Ga II states with respect to the crystal surrounding. The energy level corresponding to the metastable state Ga II is supposed to occur above the conduction band bottom, providing fast recombination rates for the negative PC. The superposition of negative and positive PC is considered to be dependent on the ratio of the densities of states corresponding to the donor and acceptor impurity centers.",0009209v1 2002-04-20,Possible Magnetic separation in Ru doped La0.67Ca0.33MnO3,"X-ray diffraction, resistivity, ac susceptibility and magnetization studies on La0.67Ca0.33Mn1-xRuxO3 (0 x < 0.1) were carried out. A significant increase in the lattice parameters indicated the presence of mixed valance state of Ru: Ru3+ and Ru4+. The resistivity of the doped compounds exhibited two features: a broad maximum and a relatively sharp peak. While a para to ferromagnetic transition could be observed for the latter peak, no magnetic signal either in ac susceptibility or in magnetization measurements could be observed for the broad maximum. The magnetic moment decreases non linearly from 3.55 to 3 mB over the Ru composition from 0 to 8.5 at.%. Based on the results of the present studies and on existing literature on the Mn-site substituted systems, we argue that a magnetic phase separation occurs in the Ru doped system. While the sharp peak in the resistivity corresponds to Ru4+ enriched region with a ferromagnetic coupling with neighboring Mn ions, the broad peak corresponds to a Ru3+ rich regions, with an antiferromagnetic coupling with neighboring Mn ions.",0204441v1 2003-02-03,Metallicity and its low temperature behavior in dilute 2D carrier systems,"We theoretically consider the temperature and density dependent transport properties of semiconductor-based 2D carrier systems within the RPA-Boltzmann transport theory, taking into account realistic screened charged impurity scattering in the semiconductor. We derive a leading behavior in the transport property, which is exact in the strict 2D approximation and provides a zeroth order explanation for the strength of metallicity in various 2D carrier systems. By carefully comparing the calculated full nonlinear temperature dependence of electronic resistivity at low temperatures with the corresponding asymptotic analytic form obtained in the $T/T_F \to 0$ limit, both within the RPA screened charged impurity scattering theory, we critically discuss the applicability of the linear temperature dependent correction to the low temperature resistivity in 2D semiconductor structures. We find quite generally that for charged ionized impurity scattering screened by the electronic dielectric function (within RPA or its suitable generalizations including local field corrections), the resistivity obeys the asymptotic linear form only in the extreme low temperature limit of $T/T_F \le 0.05$. We point out the experimental implications of our findings and discuss in the context of the screening theory the relative strengths of metallicity in different 2D systems.",0302047v3 2003-04-21,"Chemical, Structural, and Transport Properties of Na1-xCoO2","We report measurement of room-temperature compressibility, thermal expansion, thermoelectric power a(T) at various pressures P < 20 kbar, basal-plane resistivity rab (T), magnetic susceptibility and thermal conductivity k(T) taken on single-crystal or cold-pressed Na0.57CoO2. An enhancement of a large thermopower with a change of slope occurs on heating near 100 K, but this enhancement is progressively suppressed by pressure. The c-axis thermal expansion is large in the interval 150 K TQ. Moreover, in magnetic fields below 6 T, all data set of the electrical resistivity and C_4f(T) are well scaled with characteristic temperatures T0's. This is the first observation of the NFL state in the nonmagnetic quadrupole-active system, whose origin is intrinsically different from that observed in the vicinity of the conventional quantum critical point. It implies possible formation of a quadrupole Kondo lattice resulting from hybridization between the quadrupoles and the conduction electrons. Below 0.13 K, the electrical resistivity and C_4f(T) exhibit anomalies as B approaches 5 T. This is the manifestation of a field-induced crossover toward a Fermi-liquid ground state in the quadrupole Kondo lattice.",1606.09571v1 2016-10-27,Magnetoresistance and robust resistivity plateau in MoAs2,"We have grown the MoAs$_2$ single crystal which crystallizes in a monoclinic structure with C2/m space group. Transport measurements show that MoAs$_2$ displays a metallic behavior at zero field and undergoes a metal-to-semiconductor crossover at low temperatures when the applied magnetic field is over 5 T. A robust resistivity plateau appears below 18 K and persists for the field up to 9 T. A large positive magnetoresistance (MR), reaching about 2600\% at 2 K and 9 T, is observed when the field is perpendicular to the current.The MR becomes negative below 40 K when the field is rotated to be parallel to the current. The Hall resistivity shows the non-linear field-dependence below 70 K. The analysis using two-band model indicates a compensated electron-hole carrier density at low temperatures. A combination of the breakdown of Kohler's rule, the abnormal drop and the cross point in Hall data implies that a possible Lifshitz transition has occurred between 30 K and 60 K, likely driving the compensated electron-hole density, the large MR as well as the metal-semiconductor transition in MoAs$_2$. Our results indicate that the family of centrosymmetric transition-metal dipnictides has rich transport behavior which can in general exhibit variable metallic and topological features.",1610.08594v2 2017-10-24,Absence of Metallic Behavior in Epitaxial NiCo2O4 Thin Films: Role of Microstructural Disorder,"Despite the low resistivity (~ 1 mohm cm), the metallic electrical transport has not been commonly observed in the inverse spinel NiCo2O4, except in certain epitaxial thin films. Previous studies have stressed the effect of valence mixing and degree of spinel inversion on the electric conduction of NiCo2O4 films. In this work, we have studied the effect of microstructure by comparing the NiCo2O4 epitaxial films grown on MgAl2O4 (111) and on Al2O3 (0001) substrates. Although the optimal growth condition and the magnetic properties are similar for the NiCo2O4/MgAl2O4 and the NiCo2O4/Al2O3, they show metallic and semiconducting electrical transport respectively. Despite similar temperature and field dependence of magnetization, the NiCo2O4/Al2O3 show much larger magnetoresistance at low temperature. Post-growth annealing decreases the resistivity of NiCo2O4/Al2O3, but the annealed films are still semiconducting. The correlation between the structural correlation length and the resistivity suggests that the microstructural disorder, generated by the dramatic mismatch between the NiCo2O4 and Al2O3 crystal structures, may be the origin of the absence of the metallic electrical transport in NiCo2O4. These results reveal microstructural disorder as another key factor in controlling the electrical transport of NiCo2O4, with potentially large magnetoresistance for spintronics application.",1710.08608v2 2017-12-05,Peculiarities of the electronic transport in half-metallic Co-based Heusler alloys,"Electrical, magnetic and galvanomagnetic properties of half-metallic Heusler alloys of Co$_2$YZ (Y = Ti, V, Cr, Mn, Fe, Ni, and Z = Al, Si, Ga, Ge, In, Sn, Sb) were studied in the temperature range 4.2--900 K and in magnetic fields of up to 100 kOe. It was found that varying Y in affects strongly the electric resistivity and its temperature dependence $\rho(T)$, while this effect is not observed upon changing Z. When Y is varied, extrema (maximum or minimum) are observed in $\rho(T)$ near the Curie temperature $T_C$. At $T < T_C$, the $\rho(T)$ behavior can be ascribed to a change in electronic energy spectrum near the Fermi level. The coefficients of the normal and anomalous Hall effect were determined. It was shown that the latter coefficient, $R_S$, is related to the residual resistivity $\rho_0$ by a power law $R_S \sim \rho_0^k/M_S$ with $M_S$ the spontaneous magnetization. The exponent $k$ was found to be 1.8 for Co$_2$FeZ alloys, which is typical for asymmetric scattering mechanisms, and 2.9 for Co$_2$YAl alloys, which indicates an additional contribution to the anomalous Hall effect. The temperature dependence of resistivity at low temperatures is analyzed and discussed in the framework of the two-magnon scattering theory.",1712.01584v1 2017-12-25,Effects of nuclear spins on the transport properties of the edge of two-dimensional topological insulators,"The electrons in the edge channels of two-dimensional topological insulators can be described as a helical Tomonaga-Luttinger liquid. They couple to nuclear spins embedded in the host materials through the hyperfine interaction, and are therefore subject to elastic spin-flip backscattering on the nuclear spins. We investigate the nuclear-spin-induced edge resistance due to such backscattering by performing a renormalization-group analysis. Remarkably, the effect of this backscattering mechanism is stronger in a helical edge than in nonhelical channels, which are believed to be present in the trivial regime of InAs/GaSb quantum wells. In a system with sufficiently long edges, the disordered nuclear spins lead to an edge resistance which grows exponentially upon lowering the temperature. On the other hand, electrons from the edge states mediate an anisotropic Ruderman-Kittel-Kasuya-Yosida nuclear spin-spin interaction, which induces a spiral nuclear spin order below the transition temperature. We discuss the features of the spiral order, as well as its experimental signatures. In the ordered phase, we identify two backscattering mechanisms, due to charge impurities and magnons. The backscattering on charge impurities is allowed by the internally generated magnetic field, and leads to an Anderson-type localization of the edge states. The magnon-mediated backscattering results in a power-law resistance, which is suppressed at zero temperature. Overall, we find that in a sufficiently long edge the nuclear spins, whether ordered or not, suppress the edge conductance to zero as the temperature approaches zero.",1712.09040v2 2018-01-26,Local Magnetic Measurements of Trapped Flux Through a Permanent Current Path in Graphite,"Temperature and field dependent measurements of the electrical resistance of different natural graphite samples, suggest the existence of superconductivity at room temperature in some regions of the samples. To verify whether dissipationless electrical currents are responsible for the trapped magnetic flux inferred from electrical resistance measurements, we localized them using magnetic force microscopy on a natural graphite sample in remanent state after applying a magnetic field. The obtained evidence indicates that at room temperature a permanent current flows at the border of the trapped flux region. The current path vanishes at the same transition temperature $T_c\approx370$~K as the one obtained from electrical resistance measurements on the same sample. This sudden decrease of the phase is different from what is expected for a ferromagnetic material. Time dependent measurements of the signal show the typical behavior of flux creep of a permanent current flowing in a superconductor. The overall results support the existence of room-temperature superconductivity at certain regions in the graphite structure and indicate that magnetic force microscopy is suitable to localize them. Magnetic coupling is excluded as origin of the observed phase signal.",1801.08836v1 2018-01-29,Observation of the Meissner effect at room temperature in single-layer graphene brought into contact with alkanes,"There are claims of synthesis of a room temperature superconductor. However, these claims have not been officially accepted by scientific communities. Currently, the highest transition temperature (Tc) recognized in scientific articles is 135 K at 1 atm of Hg-Ba-Ca-Cu-O system which is a copper oxide superconductor. We packed graphite flakes into a ring-shaped polytetrafluoroethylene (PTFE) tube and further injected heptane or octane. Then we generated circulating current in this ring tube by electromagnetic induction and showed that this circulating current continues to flow continuously at room temperature for 50 days. This experiment suggests that bringing alkane into contact with graphite may result in a material with zero resistance at room temperature. In addition, we showed by means of AC resistance measurements using the two-terminal method that the resistances of graphite fibers brought into contact with various alkanes suddenly change at specific critical temperatures between 363 and 504 K. In this study, we show that after a magnetic field is applied to a single-layer graphene at room temperature, alkane is brought into contact with the single-layer graphene, then the graphene excludes the magnetic field immediately. This phenomenon demonstrates that the alkane-wetted single-layer graphene shows Meissner effect at room temperature. Furthermore, we applied a magnetic field perpendicularly to the annular single-layer graphene brought into contact with n-hexane and immediately removed the magnetic field. After that we observed that a constant magnetic field generates from this annular graphene for some time. In conclusion, the single-layer graphene brought into contact with alkane shows Meissner effect at room temperature, which provides definitive evidence for room temperature superconductivity.",1801.09376v1 2019-05-10,Magnetic-Field-Induced Phenomena in the Paramagnetic Superconductor UTe$_{2}$,"We present magnetoresistivity measurements on the heavy-fermion superconductor UTe$_{2}$ in pulsed magnetic fields $\mu_0H$ up to 68~T and temperatures $T$ from 1.4 to 80~K. Magnetic fields applied along the three crystallographic directions $\mathbf{a}$ (easy magnetic axis), $\mathbf{b}$, and $\mathbf{c}$ (hard magnetic axes), are found to induce different phenomena - depending on the field direction - beyond the low-field suppression of the superconducting state. For $\mathbf{H}\parallel\mathbf{a}$, a broad anomaly in the resistivity is observed at $\mu_0H^*\simeq10$~T and $T = 1.4$~K. For $\mathbf{H}\parallel\mathbf{c}$, no magnetic transition nor crossover are observed. For $\mathbf{H}\parallel\mathbf{b}$, a sharp first-order-like step in the resistivity indicates a metamagnetic transition at the field $\mu_0H_m \simeq 35$~T. When the temperature is raised signature of first-order metamagnetism is observed up to a critical endpoint at $T_{CEP}\simeq7$~K. At higher temperatures a crossover persists up to 28~K, i.e., below the temperature $T_\chi^{max} = 35$~K where the magnetic susceptibility is maximal. A sharp maximum in the Fermi-liquid quadratic coefficient $A$ of the low-temperature resistivity is found at $H_m$. It indicates an enhanced effective mass associated with critical magnetic fluctuations, possibly coupled with a Fermi surface instability. Similarly to the URhGe case, we show that UTe$_{2}$ is a candidate for field-induced reentrant superconductivity in the proximity of $H_m$.",1905.03990v1 2019-05-13,Extending Policy from One-Shot Learning through Coaching,"Humans generally teach their fellow collaborators to perform tasks through a small number of demonstrations. The learnt task is corrected or extended to meet specific task goals by means of coaching. Adopting a similar framework for teaching robots through demonstrations and coaching makes teaching tasks highly intuitive. Unlike traditional Learning from Demonstration (LfD) approaches which require multiple demonstrations, we present a one-shot learning from demonstration approach to learn tasks. The learnt task is corrected and generalized using two layers of evaluation/modification. First, the robot self-evaluates its performance and corrects the performance to be closer to the demonstrated task. Then, coaching is used as a means to extend the policy learnt to be adaptable to varying task goals. Both the self-evaluation and coaching are implemented using reinforcement learning (RL) methods. Coaching is achieved through human feedback on desired goal and action modification to generalize to specified task goals. The proposed approach is evaluated with a scooping task, by presenting a single demonstration. The self-evaluation framework aims to reduce the resistance to scooping in the media. To reduce the search space for RL, we bootstrap the search using least resistance path obtained using resistive force theory. Coaching is used to generalize the learnt task policy to transfer the desired quantity of material. Thus, the proposed method provides a framework for learning tasks from one demonstration and generalizing it using human feedback through coaching.",1905.04841v1 2019-09-18,Blockade of vortex flow by thermal fluctuations in atomically thin clean-limit superconductors,"Resistance in superconductors arises from the motion of vortices driven by flowing supercurrents or external electromagnetic fields and may be strongly affected by thermal or quantum fluctuations. The common expectation borne out in previous experiments is that as the temperature is lowered, vortex motion is suppressed, leading to a decreased resistance. A new generation of materials provides access to the previously inaccessible regime of clean-limit superconductivity in atomically thin superconducting layers. We show experimentally that for few-layer 2H-NbSe$_2$ the resistance below the superconducting transition temperature may be non-monotonic, passing through a minimum and then increasing again as temperature is decreased further. The effects exists over a wide range of current and magnetic fields, but is most pronounced in monolayer devices at intermediate currents. Analytical and numerical calculations confirm that the findings can be understood in a two-fluid vortex model, in which a fraction of vortices flow in channels while the rest are pinned but thermally fluctuating in position. We show theoretically that the pinned, fluctuating vortices effectively control the mobility of the free vortices. The findings provide a new perspective on fundamental questions of vortex mobility and dissipation in superconductors.",1909.08469v1 2019-09-19,Thermal rectification and interface thermal resistance in hybrid pillared-graphene and graphene: A molecular dynamics approach,"In this study, we investigate the thermal rectification and thermal resistance in the hybrid pillared-graphene and graphene (PGG) system. This is done through the classical molecular dynamics simulation (MD) and also with a continuum model. At first, the thermal conductivity of both pillared-graphene and graphene is calculated employing MD simulation and Fourier low. Our results show that the thermal conductivity of the pillared-graphene is much smaller than the graphene by an order of magnitude. Next, by applying positive and negative temperature gradients along the longitudinal direction of PGG, the thermal rectification is examined. The MD results indicate that for the lengths in the range of 36 to 86nm, the thermal rectification remains almost constant (~3-5%). We have also studied the phonon density of states (DOS) on both sides of the interface of PGG. The DOS curves show that there is phonon scattering at low frequencies (acoustic mode) that depends on the imposed temperature gradient direction in the system. Therefore, we can introduce the PGG as a promising thermal rectifier at room temperature. Furthermore, in the following of this work, we also explore the temperature distribution over the PGG by using the continuum model. The results that obtained from the continuum model predict the MD results such as the temperature distribution in the upper half layer and lower full layer graphene, the temperature gap and also the thermal resistance at the interface.",1909.08971v1 2014-08-19,"Device Perspective for Black Phosphorus Field-Effect Transistors: Contact Resistance, Ambipolar and Scaling","Although monolayer black phosphorus (BP) or phosphorene has been successfully exfoliated and its optical properties have been explored, most of electrical performance of the devices is demonstrated on few-layer phosphorene and ultra-thin BP films. In this paper, we study the channel length scaling of ultra-thin BP field-effect transistors (FETs), and discuss a scheme for using various contact metals to change transistor characteristics. Through studying transistor behaviors with various channel lengths, the contact resistance can be extracted from the transfer length method (TLM). With different contact metals, we find out that the metal/BP interface has different Schottky barrier heights, leading to a significant difference in contact resistance, which is quite different from previous studies of transition metal dichalcogenides (TMDs) such as MoS2 where Fermi-level is strongly pinned near conduction band edge at metal/MoS2 interface. The nature of BP transistors are Schottky barrier FETs, where the on and off states are controlled by tuning the Schottky barriers at the two contacts. We also observe the ambipolar characteristics of BP transistors with enhanced n-type drain current and demonstrate that the p-type carriers can be easily shifted to n-type or vice versus by controlling the gate bias and drain bias, showing the potential to realize BP CMOS logic circuits.",1408.4206v2 2014-08-19,Exploring quantum phase transition in Pd_{1-x}Ni_x nanoalloys,"Pd$_{1-x}$Ni$_x$ alloy system is an established ideal transition metal system possessing a composition induced paramagnetic to ferromagnetic quantum phase transition (QPT) at the critical concentration $x_c \sim$ 0.026 in bulk. A low-temperature non-Fermi liquid (NFL) behaviour around $x_c$ usually indicates the presence of quantum criticality (QC) in this system. In this work, we explore the existence of such a QPT in nanoparticles of this alloy system. We synthesized single-phase, polydispersed and 40-50 nm mean diameter crystalline nanoparticles of Pd$_{1-x}$Ni$_x$ alloys, with $x$ near $x_c$ and beyond, by a chemical reflux method. In addition to the determination of the size, composition, phase and crystallinity of the alloys by microscopic and spectroscopic techniques, the existence of a possible QPT was explored by resistivity and DC magnetization measurements. A dip in the value of the exponent $n$ near $x_c$, and a concomitant peak in the constant $A$, of the $AT^n$ dependence of the low temperature ($T$) resistivity indicate the presence of a quantum-like phase transition in the system. The minimum value of $n$, however, remains within the Fermi liquid regime ($n >$ 2). The DC magnetization results suggest an anticipatory presence of a superparamagnetic to ferromagnetic QPT in the mean-sized nanoparticles. The observation of a possible quantum critical NFL behaviour ($n <$ 2) through resistivity is argued to be inhibited by the electron-magnon scatterings present in the smaller nanoparticles.",1408.4316v1 2017-01-03,Conduction Channel Formation and Dissolution Due to Oxygen Thermophoresis/Diffusion in Hafnium Oxide Memristors,"Transition metal oxide memristors, or resistive random-access memory (RRAM) switches, are under intense development for storage-class memory because of their favorable operating power, endurance, speed, and density. Their commercial deployment critically depends on predictive compact models based on understanding nanoscale physico-chemical forces, which remains elusive and controversial owing to the difficulties in directly observing atomic motions during resistive switching, Here, using scanning transmission synchrotron x-ray spectromicroscopy to study in-situ switching of hafnium oxide memristors, we directly observed the formation of a localized oxygen-deficiency-derived conductive channel surrounded by a low-conductivity ring of excess oxygen. Subsequent thermal annealing homogenized the segregated oxygen, resetting the cells towards their as-grown resistance state. We show that the formation and dissolution of the conduction channel are successfully modeled by radial thermophoresis and Fick diffusion of oxygen atoms driven by Joule heating. This confirmation and quantification of two opposing nanoscale radial forces that affect bipolar memristor switching are important components for any future physics-based compact model for the electronic switching of these devices.",1701.00864v1 2018-10-05,Effect of impurities on morphology and growth mode of (111) and (001) epitaxial-like ScN films,"ScN material is an emerging semiconductor with an indirect bandgap. It has attracted attention for its thermoelectric properties, use as seed layers, and for alloys for piezoelectric application. ScN or other transition metal nitride semiconductors used for their interesting electrical properties are sensitive to contaminants, such as oxygen or fluorine. In this present article, the influence of depositions conditions on the amount of oxygen contaminants incorporated in ScN films were investigated and their effects on the electrical properties (electrical resistivity and Seebeck coefficient) were studied. The epitaxial-like films of thickness 125 +-5 nm to 155 +-5 nm were deposited by D.C.-magnetron sputtering on c-plane Al2O3, MgO(111) and r-plane Al2O3 at a substrate temperature ranging from 700 to 950 degree C. The amount of oxygen contaminants presents in the film, dissolved into ScN or as an oxide, was related to the adatom mobility during growth, which is affected by the deposition temperature and the presence of twin domain growth. The lowest values of electrical resistivity of 50 micro-ohm cm were obtained on ScN(111)/MgO(111) and on ScN(001)/r-plane Al2O3 grown at 950 degree C with no twin domains and the lowest amount of oxygen contaminant. At the best, the films exhibited an electrical resistivity of 50 micro-ohm cm with Seebeck coefficient values maintained at -40 microV K-1, thus a power factor estimated at 3.2 10-3 W m-1 K-2 (at room temperature).",1810.02593v1 2019-07-05,A post mortem analysis of the strain-induced crystallization effects on fatigue of elastomers,"Natural rubber (NR) is the most commonly used elastomer in the automotive industry thanks to its outstanding fatigue resistance. Strain-induced crystallization (SIC) is found to play a role of paramount importance in the great crack growth resistance of NR [1]. Typically, NR exhibits a lifetime reinforcement for non-relaxing loadings [2-3]. At the microscopic scale, fatigue striations were observed on the fracture surface of Diabolo samples tested in fatigue. They are the signature of SIC [2,4,5]. In order to provide additional information on the role of SIC in the fatigue crack growth resistance of NR, striations are investigated through post-mortem analysis after fatigue experiments using loading ranging from-0.25 to 0.25. No striation was observed in the case of tests performed at 90{\textdegree}C. This confirms that the formation of striation requires a certain crystallinity level in the material. At 23{\textdegree}C, two striation regimes were identified: small striation patches with different orientations (Regime 1) and zones with large and well-formed striations (Regime 2). Since fatigue striations are observed for all the loading ratios applied, they are therefore not the signature of the reinforcement. Nevertheless, increasing the minimum value of the strain amplified the striation phenomenon and the occurrence of Regime 2.",1907.02688v1 2022-02-12,Expansion of Graphene-Based Device Technology for Resistance Metrology,"The field of Quantum Hall metrology had a strong start with the implemntation of GaAs-based devices, given that 2D materials systems provided access to interesting quantum phenomena, including the infrastructure associated with making relevant measurements. With the technology laid out, further improvements in both infrastructure and standards were achieved in the previous two decades as EG-based quantized Hall resistance (QHR) devices became established as national standards. Since the metrology community has reached some understanding that a comparison against GaAs-based QHR devices had been accomplished, the next steps became clearer as far as how the EG-based QHR with a single Hall bar could be further developed. Since the early 90s, it has been of modest interest that QHR devices have a means of interconnecting several single Hall bar elements and has since been a subject of research. NMIs are now presently at a juncture where consideration must be granted beyond just simplicity of operation. A natural direction for resistance standards would be to increase the total accessible parameter space. This means using EG-based QHR devices to output more than the single value at the $\nu = 2$ plateau (about 12.9 k$\Omega$). A first natural question is whether one may use the $\nu = 6$ plateau or $\nu = 10$ plateau, and though some work has been done with these Landau levels in graphene, they simply do not offer the same level of precision as the $\nu = 2$ plateau.",2202.05954v1 2016-03-21,Influence of rhombohedral stacking order in the electrical resistance of bulk and mesoscopic graphite,"The electrical, in-plane resistance as a function of temperature $R(T)$ of bulk and mesoscopic thin graphite flakes obtained from the same batch was investigated. Samples thicker than $\sim 30$ nm show metalliclike contribution in a temperature range that increases with the sample thickness, whereas a semiconductinglike behavior was observed for thinner samples. The temperature dependence of the in-plane resistance of all measured samples and several others from literature can be very well explained between 2 K and 1100 K assuming three contributions in parallel: a metalliclike conducting path at the interfaces between crystalline regions, composed of two semiconducting phases, i.e. Bernal and rhombohedral stacking. From the fits of $R(T)$ we obtain a semiconducting energy gap of $110 \pm 20$meV for the rhombohedral and $38\pm 8 $meV for the Bernal phase. The presence of these crystalline phases was confirmed by x-ray diffraction measurements. We review similar experimental data from literature of the last 33 years and two more theoretical models used to fit $R(T)$.",1603.06365v3 2017-04-03,Plasmonic heating in Au nanowires at low Temperatures: The role of thermal boundary resistance,"Inelastic electron tunneling and surface-enhanced optical spectroscopies at the molecular scale require cryogenic local temperatures even under illumination - conditions that are challenging to achieve with plasmonically resonant metallic nanostructures. We report a detailed study of the laser heating of plasmonically active nanowires at substrate temperatures from 5 to 60 K. The increase of the local temperature of the nanowire is quantified by a bolometric approach and could be as large as 100 K for a substrate temperature of 5 K and typical values of laser intensity. We also demonstrate that a $\sim 3\times$ reduction of the local temperature increase is possible by switching to a sapphire or quartz substrate. Finite element modeling of the heat dissipation reveals that the local temperature increase of the nanowire at temperatures below $\sim$50 K is determined largely by the thermal boundary resistance of the metal-substrate interface. The model reproduces the striking experimental trend that in this regime the temperature of the nanowire varies nonlinearly with the incident optical power. The thermal boundary resistance is demonstrated to be a major constraint on reaching low temperatures necessary to perform simultaneous inelastic electron tunneling and surface enhanced Raman spectroscopies.",1704.00771v1 2017-05-18,Effects of the Functional Group on the Lithium Ions Across the Port of Carbon Nanotube,"The mean axial velocity of lithium irons across the entrance of carbon nanotube VLi is an important factor for the charge-discharge performances of rechargeable Lithium battery. The molecular dynamics simulation method is adopted to evaluate the factors and their effects on VLi which include the diameter of carbon nanotube, functional group type on the port and the number of a given type of functional group. The statistical analysis of the calculation results shows that: In the selected carbon nanotubes of four different diameters, VLi will gradually rise with the increase of CNT diameter due to lithium irons migration resistance decreasing; as the port of CNT is successively modified to hydrogen (-H), hydroxyl (-OH), amino (-NH2) and carboxyl (-COOH), the corresponding migration resistance of lithium ions is enhanced resulting in the dropping of VLi; in comparison to the effect strength of four types of functional groups on VLi, -COOH shows strongest, -NH2 and -OH perform relatively weaker, and the effect difference between -NH2 and -OH is very small, -H displays weakest; When the number of a given non-hydrogen functional group on the port sequentially increases, it also shows a trend that lithium ion migration resistance gradually increases which makes VLi decreases in turn. The more influential the functional group, the greater the impact of functional group number changes on VLi. The results of this paper have some significance on the precise production of lithium-ion battery electrode materials, enhancing the overall battery cycle efficiency and charging speed.",1705.06650v1 2017-08-24,Memory matrix theory of the dc resistivity of a disordered antiferromagnetic metal with an effective composite operator,"We perform the calculation of the dc resistivity as a function of temperature of the ""strange-metal"" state that emerges in the vicinity of a spin-density-wave phase transition in the presence of weak disorder. This scenario is relevant to the phenomenology of many important correlated materials, such as, e.g., the pnictides, the heavy-fermion compounds and the cuprates. To accomplish this task, we implement the memory-matrix approach that allows the calculation of the transport coefficients of the model beyond the quasiparticle paradigm. Our computation is also inspired by the $\epsilon=3-d$ expansion in a hot-spot model embedded in $d$-space dimensions recently put forth by Sur and Lee [Phys. Rev. B 91, 125136 (2015)], in which they find a new low-energy non-Fermi liquid fixed point that is perturbatively accessible near three dimensions. As a consequence, we are able to establish here the temperature and doping dependence of the electrical resistivity at intermediate temperatures of a two-dimensional disordered antiferromagnetic metallic model with a composite operator that couples the order-parameter fluctuations to the entire Fermi surface. We argue that our present theory provides a good basis in order to unify the experimental transport data, e.g., in the cuprates and the pnictide superconductors, within a wide range of doping regimes.",1708.07537v1 2019-04-03,Patterning of diamond like carbon films for sensor applications using silicon containing thermoplastic resist (SiPol) as a hard mask,"Patterning of diamond-like carbon (DLC) and DLC:metal nanocomposites is of interest for an increasing number of applications. We demonstrate a nanoimprint lithography process based on silicon containing thermoplastic resist combined with plasma etching for straightforward patterning of such films. A variety of different structures with few hundred nanometer feature size and moderate aspect ratios were successfully realized. The quality of produced patterns was directly investigated by the means of optical and scanning electron microscopy (SEM). Such structures were further assessed by employing them in the development of gratings for guided mode resonance (GMR) effect. Optical characterization of such leaky waveguide was compared with numerical simulations based on rigorous coupled wave analysis method with good agreement. The use of such structures as refractive index variation sensors is demonstrated with sensitivity up to 319 nm/RIU, achieving an improvement close to 450% in sensitivity compared to previously reported similar sensors. This pronounced GMR signal fully validates the employed DLC material, the technology to pattern it and the possibility to develop DLC based gratings as corrosion and wear resistant refractometry sensors that are able to operate under harsh conditions providing great value and versatility.",1904.01880v1 2019-04-02,Filament mechanics in a half-space via regularised Stokeslet segments,"We present a generalisation of efficient numerical frameworks for modelling fluid-filament interactions via the discretisation of a recently-developed, non-local integral equation formulation to incorporate regularised Stokeslets with half-space boundary conditions, as motivated by the importance of confining geometries in many applications. We proceed to utilise this framework to examine the drag on slender inextensible filaments moving near a boundary, firstly with a relatively-simple example, evaluating the accuracy of resistive force theories near boundaries using regularised Stokeslet segments. This highlights that resistive force theories do not accurately quantify filament dynamics in a range of circumstances, even with analytical corrections for the boundary. However, there is the notable and important exception of movement in a plane parallel to the boundary, where accuracy is maintained. In particular, this justifies the judicious use of resistive force theories in examining the mechanics of filaments and monoflagellate microswimmers with planar flagellar patterns moving parallel to boundaries. We proceed to apply the numerical framework developed here to consider how filament elastohydrodynamics can impact drag near a boundary, analysing in detail the complex responses of a passive cantilevered filament to an oscillatory flow. In particular, we document the emergence of an asymmetric periodic beating in passive filaments in particular parameter regimes, which are remarkably similar to the power and reverse strokes exhibited by motile 9+2 cilia. Furthermore, these changes in the morphology of the filament beating, arising from the fluid-structure interactions, also induce a significant increase in the hydrodynamic drag of the filament.",1904.02543v2 2015-07-23,Spatially resolved TiOx phases in RRAM conductive nanofilaments using soft X-ray spectromicroscopy,"Reduction in metal-oxide thin films has been suggested as the key mechanism responsible for forming conductive nanofilaments within solid-state memory devices, enabling their resistive switching capacity. The quantitative spatial identification of such filaments is a daunting task, particularly for metal-oxides capable of exhibiting multiple phases as in the case of TiOx. Here, we spatially resolve and chemically characterize distinct TiOx phases in localized regions of a TiOx-based memristive device by combining full-field transmission X-ray microscopy with soft X-ray spectroscopic analysis that is performed on lamella samples. We particularly show that electrically pre-switched devices in low-resistive states comprise reduced disordered phases with O/Ti ratios close to Ti2O3 stoichiometry that aggregate in a ~ 100 nm filamentary region electrically conducting the top and bottom electrodes of the devices. We have also identified crystalline rutile and orthorhombic-like TiO2 phases in the region adjacent to the filament, suggesting that the temperature increases locally up to 1000 K, validating the role of Joule heating in resistive switching. Contrary to previous studies, our approach enables to simultaneously investigate morphological and chemical changes in a quantitative manner without incurring difficulties imposed by interpretation of electron diffraction patterns acquired via conventional electron microscopy techniques.",1507.06588v1 2019-01-16,Quantum oscillations in strongly correlated topological Kondo insulators,"The observation of quantum oscillations in topological Kondo insulators SmB6 and YbB12 is a recent puzzling experimental discovery. Quantum oscillations observed in the resistivity and the magnetization are usually explained by the existence of the Fermi surface. However, Kondo insulators do not have a Fermi surface and thus should not show quantum oscillations. By performing dynamical mean-field calculations for topologically nontrivial Kondo insulators in a magnetic field, we analyze the effect of correlations on the emergence of quantum oscillations in narrow-gap topological Kondo insulators and demonstrate that the interplay between correlations and nonlocal hybridization, ubiquitously occurring in topological Kondo insulators, can lead to observable quantum oscillations without the necessity of a Fermi surface. Particularly, we show that correlations make it easier to observe quantum oscillations in the magnetization and the resistivity of the bulk material. The fundamental mechanism for these quantum oscillations is a combination of correlation effects and Landau levels coming very close to the Fermi energy. We furthermore demonstrate that quantum oscillations in a three-dimensional system can be understood by analyzing the physics on the two-dimensional planes in the momentum space for which the hybridization in direction of the magnetic field vanishes. We believe that this scenario is relevant to understanding the observation of quantum oscillations in the magnetic torque for SmB6 as well as oscillations in the resistivity and the magnetic torque of YbB12.",1901.05099v2 2019-10-18,Probing quantum spin liquids in equilibrium using the inverse spin Hall effect,"We propose an experimental method utilizing a strongly spin-orbit coupled metal to quantum magnet bilayer that will probe quantum magnets lacking long range magnetic order, e.g., quantum spin liquids, via examination of the voltage noise spectrum in the metal layer. The bilayer is held in thermal and chemical equilibrium, and spin fluctuations arising across the single interface are converted into voltage fluctuations in the metal as a result of the inverse spin Hall effect. We elucidate the theoretical workings of the proposed bilayer system, and provide precise predictions for the frequency characteristics of the enhancement to the ac electrical resistance measured in the metal layer for three candidate quantum spin liquid models. Application to the Heisenberg spin-$1/2$ kagom{\'e} lattice model should allow for the extraction of any spinon gap present. A quantum spin liquid consisting of fermionic spinons coupled to a $U(1)$ gauge field should cause subdominant $\W^{4/3}$ scaling of the resistance of the coupled metal. Finally, if the magnet is well-captured by the Kitaev model in the gapless spin liquid phase, then the proposed bilayer can extract the two-flux gap which arises in spite of the gapless spectrum of the fermions. We therefore show that spectral analysis of the ac resistance in the metal in a single interface, equilibrium bilayer can test the relevance of a quantum spin liquid model to a given candidate material.",1910.08610v2 2020-05-23,Mixed ground state in Fe-Ni Invar alloys,"We investigate the ground state properties of Invar alloys via detailed study of the electronic structure of Fe$_{1-x}$Ni$_x$ alloys ($x$ = 0.2, 0.3, 0.4, 0.5, 0.6, 0.7, 0.9) employing $x$-ray photoelectron spectroscopy (XPS). While all the alloys exhibit soft ferromagnetic behavior with Curie temperature much higher than the room temperature, the results for invar alloy, Fe$_{0.6}$Ni$_{0.4}$ exhibit anomalous behavior. Moreover, the magneto-resistance of the Invar alloy becomes highly negative while the end members possess positive magneto-resistance. The core level spectra of the Invar alloy exhibit emergence of a distinct new feature below 20~K while all other Fe-Ni alloys exhibit no temperature dependence down to 10~K. Interestingly, the shallow core level spectra (3$s$, 3$p$) of Fe and Ni of the Invar alloy reveal stronger deviation at low temperatures compared to the deep core levels (2$s$, 2$p$) indicating crystal field effect. It appears that there is a large precipitation of antiferromagnetic $\gamma^\prime$ phase below 20 K possessing low magnetic moment (0.5$\mu_B$) on Fe within the $\alpha$ phase. The discovery of negative magneto-resistance, anomalous magnetization at low temperature and the emergence of unusual new features in the core levels at low temperature provide an evidence of mixed phase in the ground state of Invar alloys.",2005.11493v1 2020-07-01,"Impact of V substitution on the physical properties of Ni-Zn-Co ferrites: structural, magnetic, dielectric and electrical properties","We have investigated the Vanadium- (V) substituted Ni-Zn-Co ferrites where the samples were prepared using solid-state reaction technique. The impact of V5+ substitution on the structural, magnetic, dielectric and electrical properties of Ni-Zn-Co ferrites has been studied. XRD analysis confirmed the formation of a single-phase cubic spinel structure. The lattice constants have been calculated both theoretically and experimentally along with other structural parameters such as bulk density, X-ray density and porosity. The FESEM images are taken to study the surface morphology. FTIR measurement is also performed which confirms spinel structure formation. The saturation magnetization (Ms), coercive field (Hc) and Bohr magneton (B) were calculated from the obtained M-H loops. The temperature dependent permeability is studied to obtain the Curie temperature. Frequency and composition dependence of permeability was also analyzed. Dielectric behavior and ac resistivity are also subjected to investigate the frequency dependency. An inverse relationship was observed between the composition dependence of dielectric constant and ac resistivity. The obtained results such as the electrical resistivity, dielectric constants and magnetic properties suggest the appropriateness of the studied ferrites in microwave device applications.",2007.00602v1 2020-07-20,Capping and gate control of anomalous Hall effect and hump structure in ultra-thin SrRuO$_3$ films,"Ferromagnetism and exotic topological structures in SrRuO$_3$ (SRO) induce sign-changing anomalous Hall effect (AHE). Recently, hump structures have been reported in the Hall resistivity of SRO thin films, especially in the ultra-thin regime. We investigate the AHE and hump structure in the Hall resistivity of SRO ultra-thin films with an SrTiO$_3$ (STO) capping layer and ionic liquid gating. STO capping results in sign changes in the AHE and modulation of the hump structure. In particular, the hump structure in the Hall resistivity is strongly modulated and even vanishes in STO-capped 4 unit cell (uc) films. In addition, the conductivity of STO-capped SRO ultra-thin films is greatly enhanced with restored ferromagnetism. We also performed ionic liquid gating to modulate the electric field at SRO/STO interface. Drastic changes in the AHE and hump structure are observed with different gate voltages. Our study shows that the hump structure as well as the AHE can be controlled by tuning inversion symmetry and the electric field at the interface.",2007.09872v2 2020-07-23,Origin of gap-like behaviors in URu$_2$Si$_2$: Combined study via quasiparticle scattering spectroscopy and resistivity measurements,"We address two long-standing questions regarding the hidden order in URu2Si2: Is it associated with the hybridization process, and what are the distinct roles played by the localized and itinerant electrons? Our quasiparticle scattering spectroscopy reveals a hybridization gap ubiquitous in the entire phase space spanned by P and Fe substitutions in URu2Si2, including the no-order and antiferromagnetic regions, with minimal change upon crossing the phase boundary. This indicates its opening isn't associated with the ordering, and thus localized electrons must be the major player. Towards a consistent understanding of all the other gap-like behaviors observed only below transition temperatures, we analyze the electrical resistivity using a model in which gapped bosonic excitations are the dominant scattering source. With their stiffness set to follow an unusual temperature dependence (decreasing with decreasing temperature), this model fits all of our resistivity data well including the jump at the transition. Remarkably, the extracted gap increases slowly with increasing Fe content, similarly to the gap detected by inelastic neutron scattering at Q1 = (1.4, 0, 0), suggesting a common origin. Such a model can also naturally explain the Hall effect temperature dependence without invoking Fermi surface gapping.",2007.12235v2 2020-10-11,Hydrothermal synthesis and complete phase diagram of FeSe$_{1-x}$S$_{x}$ $(0 \leq x \leq 1)$ single crystals,"We report the successful synthesis of FeSe$_{1-x}$S$_{x}$ single crystals with $x$ ranging from 0 to 1 via a hydrothermal method. A complete phase diagram of FeSe$_{1-x}$S$_{x}$ has been obtained based on resistivity and magnetization measurements. The nematicity is suppressed with increasing $x$, and a small superconducting dome appears within the nematic phase. Outside the nematic phase, the superconductivity is continuously suppressed and reaches a minimum $T_c$ at $x$ = 0.45; beyond this point, $T_c$ slowly increases until $x$ = 1. Intriguingly, an anomalous resistivity upturn with a characteristic temperature $T^*$ in the intermediate region of $0.31 \leq x \leq 0.71$ is observed. $T^{*}$ shows a dome-like behavior with a maximum value at $x$ = 0.45, which is opposite the evolution of $T_c$, indicating competition between $T^*$ and superconductivity. The origin of $T^*$ is discussed in detail. Furthermore, the normal state resistivity evolves from non-Fermi-liquid to Fermi-liquid behavior with S doping at low temperatures, accompanied by a reduction in electronic correlations. Our study addresses the lack of single crystals in the high-S doping region and provides a complete phase diagram, which will promote the study of relations among nematicity, superconductivity, and magnetism.",2010.05191v3 2021-03-12,Area-selective deposition and B $δ$-doping of Si(100) with BCl$_{3}$,"B-doped $\delta$-layers were fabricated in Si(100) using BCl$_{3}$ as a dopant precursor in ultrahigh vacuum. BCl$_{3}$ adsorbed readily at room temperature, as revealed by scanning tunneling microscopy (STM) imaging. Annealing at elevated temperatures facilitated B incorporation into the Si substrate. Secondary ion mass spectrometry (SIMS) depth profiling demonstrated a peak B concentration $>$ 1.2(1) $\times$ 10$^{21}$ cm$^{-3}$ with a total areal dose of 1.85(1) $\times$ 10$^{14}$ cm$^{-2}$ resulting from a 30 L BCl$_{3}$ dose at 150 $^{\circ}$C. Hall bar measurements of a similar sample were performed at 3.0 K revealing a sheet resistance of $R_{\mathrm{s}}$ = 1.91 k$\Omega\square^{-1}$, a hole concentration of $n$ = 1.90 $\times$ 10$^{14}$ cm$^{-2}$ and a hole mobility of $\mu$ = 38.0 cm$^{2}$V$^{-1}$s$^{-1}$ without performing an incorporation anneal. Further, the conductivity of several B-doped $\delta$-layers showed a log dependence on temperature suggestive of a two-dimensional system. Selective-area deposition of BCl$_{3}$ was also demonstrated using both H- and Cl-based monatomic resists. In comparison to a dosed area on bare Si, adsorption selectivity ratios for H and Cl resists were determined by SIMS to be 310(10):1 and 1529(5):1, respectively, further validating the use of BCl$_{3}$ as a dopant precursor for atomic precision fabrication of acceptor-doped devices in Si.",2103.07529v1 2021-05-21,"Convection, Heat Generation and Particle Deposition in Direct Laser Writing of Metallic Microstructures","Three-dimensional metallic microstructures find applications as stents in medicine, as ultrabroadband antennas in communications, in micromechanical parts or as structures of more fundamental interest in photonics like metamaterials. Direct metal printing of such structures using three-dimensional laser lithography is a promising approach, which is not extensively applied yet, as fabrication speed, surface quality, and stability of the resulting structures are limited so far. In order to identify the limiting factors, we investigate the influence of light-particle interactions and varying scan speed on heat generation and particle deposition in direct laser writing of silver. We introduce a theoretical model which captures diffusion of particles and heat as well as the fluid dynamics of the photo-resist. Chemical reactions are excluded from the model but particle production is calibrated using experimental data. We find that optical forces generally surmount those due to convection of the photo-resist. Simulations predict overheating of the photo-resist at laser powers similar to those found in experiments. The thermal sensitivity of the system is essentially determined by the largest particles present in the laser focus. Our results suggest that to improve particle deposition and to achieve higher writing speeds in metal direct laser writing, strong optical trapping of the emerging particles is desirable. Furthermore, precise control of the particle size reduces the risk of spontaneous overheating.",2105.10243v2 2021-10-29,Optimal asymmetry of transistor-based terahertz detectors,"Detectors of terahertz radiation based on field-effect transistors (FETs) are among most promising candidates for low-noise passive signal rectification both in imaging systems and wireless communications. However, it was not realised so far that geometric asymmetry of common FET with respect to source-drain interchange is a strong objective to photovoltage harvesting. Here, we break the traditional scheme and reveal the optimally-asymmetric FET structure providing the maximization of THz responsivity. We fabricate a series of graphene transistors with variable top gate position with respect to mid-channel, and compare their sub-THz responsivities in a wide range of carrier densities. We show that responsivity is maximized for input gate electrode shifted toward the source contact. Theoretical simulations show that for large channel resistance, exceeding the gate impedance, such recipe for responsivity maximisation is universal, and holds for both resistive self-mixing and photo-thermoelectric detection pathways. In the limiting case of small channel resistance, the thermoelectric and self-mixing voltages react differently upon changing the asymmetry, which may serve to disentangle the origin of nonlinearities in novel materials.",2110.15810v1 2021-12-06,"Dynamical Mean Field Theory of Moiré Bilayer Transition Metal Dichalcogenides: Phase Diagram, Resistivity, and Quantum Criticality","We present a comprehensive dynamical mean field study of the triangular lattice moir\'e Hubbard model, which is believed to represent the physics of moir\'e bilayer transition metal dichalcogenides. In these materials, important aspects of the band structure including the bandwidth and the order and location of van Hove singularities can be tuned by varying the interlayer potential. We present a magnetic and metal-insulator phase diagram and a detailed study of the dependence of the resistivity on temperature, band filling and interlayer potential. We find that transport displays Fermi liquid, strange metal and quantum critical behaviors in distinct regions of the phase diagram. Specifically, we find that the cube-root van Hove singularity ($\rho(\epsilon) \sim|\epsilon|^{-1 / 3}$) gives a strange metal behavior with a $T$-linear scattering rate and $\omega/T$ scaling. We show how magnetic order affects the resistivity. Our results elucidate the physics of the correlated states and the metal-insulator continuous transition recently observed in twisted homobilayer WSe$_2$ and heterobilayer MoTe$_2$/WSe$_2$ experiments.",2112.03080v3 2022-03-15,Challenges and opportunities of srf theory for next generation particle accelerators,"We suggest a program to establish theoretical performance limits of srf cavities using modern theories of nonequilibrium superconductivity under a strong electromagnetic field. These theories will be used to calculate the main parameter of merit of srf cavities: the quality factor Q and its dependencies on the field amplitude, temperature and frequency, which would allow us to understand how far the srf cavity performance could be pushed from the current state of the art. Given that the quality factor is determined by multiple mechanisms operating on very different length scales, we will address the interconnected problems of a nonlinear surface resistance, rf losses of vortices trapped in the cavity, the effect of materials defects and surface topography, and the opportunities to boost the srf performance by surface nano-structuring, impurity management and multilayers. We suggest the following directions of theoretical srf research to address the goals of boosting the performance of the next generation particle accelerators: 1. Establishing the Q limit, mechanisms of nonlinear surface resistance and the residual resistance in a nonequilibrium superconductor under a strong RF field. 2. Establishing the srf breakdown field limit, dynamic superheating field and its dependencies on frequency, temperature and concentration of impurities. 3. Losses due to trapped vortices and extreme dynamics of ultrafast vortices driven by strong rf Meissner currents in srf cavities. 4. Optimization of srf performance due to surface nanostructuring of the cavity surface, multilayers and impurity management.",2203.08315v1 2022-05-19,Electrical Circuit Modelling of Nanofluidic Systems,"Nanofluidic systems exhibit transport characteristics that have made technological marvels such as desalination, energy harvesting, and highly sensitive biomolecule sensing possible by virtue of their ability to influence small currents due to the selective transport of ions. Traditionally many of these applications have relied on the use of nanoporous membranes. The immense complexities of membrane geometry often impede a comprehensive understanding of the underlying physics. To bypass the associated difficulties, here we consider the much simpler nanochannel array comprised of numerous nanochannels and elucidate the effects of interchannel interactions on the Ohmic response of the array. We demonstrate that a nanochannel array is equivalent to an array of mutually independent but identical unit-cells whereby the array can be represented by an equivalent electrical circuit of unit-cell resistances connected in a parallel configuration. We show that the total resistance of the system scales inversely to the number of channels. We further deconstruct the unit-cell to be a combination of multiple contributing resistances connected in series. We validate the theoretical model underlying these electrical abstractions using numerical simulations and experiments. Our approach to modeling realistic nanofluidic systems by their equivalent electrical circuit provides an invaluable tool for analyzing and interpreting experimental measurements, characterization of surface charge properties of newly developed materials, and a method for the design and development of function-specific nanofluidic devices.",2205.09437v3 2022-06-08,Phonon-limited resistivity of multilayer graphene systems,"We calculate the theoretical contribution to the doping and temperature ($T$) dependence of electrical resistivity due to scattering by acoustic phonons in Bernal bilayer graphene (BBG) and rhombohedral trilayer graphene (RTG). We focus on the role of nontrivial geometric features of the detailed, anisotropic $k\cdot p$ band structures of these systems - e.g. Van Hove singularities, Lifshitz transitions, Fermi surface anisotropy, and band curvature near the gap - whose effects on transport have not yet been systematically studied. We find that these geometric features strongly influence the temperature and doping dependencies of the resistivity. In particular, the band geometry leads to a nonlinear $T$-dependence in the high-$T$ equipartition regime, complicating the usual $T^4$ to $T$ Bloch-Gr\""{u}neisen crossover. Our focus on BBG and RTG is motivated by recent experiments in these systems that have discovered several exotic low-$T$ superconductivity proximate to complicated hierarchies of isospin-polarized phases. These interaction-driven phases are intimately related to the geometric features of the band structures, highlighting the importance of understanding the influence of band geometry on transport. While resolving the effects of the anisotropic band geometry on the scattering times requires nontrivial numerical solution, our approach is rooted in intuitive Boltzmann theory. We compare our results with recent experiment and discuss how our predictions can be used to elucidate the relative importance of various scattering mechanisms in these systems.",2206.04080v2 2022-07-18,Confinement-Induced Chiral Edge Channel Interaction in Quantum Anomalous Hall Insulators,"In quantum anomalous Hall (QAH) insulators, the interior is insulating but electrons can travel with zero resistance along one-dimensional conducting paths known as chiral edge channels (CECs). These CECs have been predicted to be confined to the one-dimensional (1D) edges and exponentially decay in the two-dimensional (2D) bulk. In this work, we present the results of a systematic study of QAH devices fashioned in a Hall bar geometry of different widths. At the charge neutral point, the QAH effect persists in a Hall bar device with a width of only ~72 nm, implying the intrinsic decaying length of CECs is less than ~36 nm. In the electron-doped regime, we find that the Hall resistance deviates quickly from the quantized value when the sample width is less than 1 um. Our theoretical calculations suggest that the deviation from the quantized Hall resistance in narrow QAH samples originates from the interaction between two opposite CECs mediated by disorder-induced bulk states in QAH insulators, consistent with our experimental observations.",2207.08371v1 2022-09-12,Robust design optimization for enhancing delamination resistance of composites,"Recent developments in the field of computational modeling of fracture have opened up possibilities for designing structures against failure. A special case, called interfacial fracture or delamination, can occur in loaded composite structures where two or more materials are bonded together at comparatively weak interfaces. Due to the potential crack growth along these interfaces, the structural problem suffers from snap-back/snap-through instabilities and bifurcations with respect to the model parameters, leading to noisy and discontinuous responses. For such a case, the design optimization problem for a selected quantity of interest is ill-posed, since small variations in the design parameters can lead to large jumps in the structural response. To this end, this paper presents a stochastic optimization approach to maximize delamination resistance that is less sensitive to small perturbations of the design and thereby leads to a robust solution. To overcome the intractability of Monte Carlo methods for estimating the expected value of the expensive-to-evaluate response function, a global, piecewise-constant surrogate is constructed based on nearest-neighbor interpolation that is iteratively refined during the optimization run. We found that by taking a large stochastic region at the beginning of the optimization and gradually reducing it to the desired one can help overcome poor local optima. Our results demonstrate the effectiveness of the proposed framework using an example of shape optimization of hard inclusions embedded in a double-cantilever beam, which significantly enhances delamination resistance.",2209.05241v1 2022-10-25,Enhanced Thermoelectric Performance of Nanostructured Nickel Doped Ag2Te,"We report on the thermoelectric properties of nickel doped Ag2-xNixTe (x = 0, 0.015, 0.025 & 0.055, 0.115, 0.155) nanostructures in the temperature (T) range of 5 K to 575 K. The electrical resistivity of Ag2Te nanostructure shows metallic behaviour in 5 K to 300 K initially that evolves into two metal to insulator transitions (MITs) at low and mid-temperature regimes with increasing x due to Mott-variable range hopping (VRH) and Arrhenius transports, respectively. Their Seebeck coefficient varies nearly in a linear fashion in this temperature range, showing metallic or doped-degenerate semiconducting behaviour. Notably, this behaviour of the Seebeck coefficient is in contrast to Mott VRH conduction as observed in resistivity. The steady increase in resistivity and S with the sharp decrease in thermal conductivity between 410 K to 425 K associated with the structural phase transition accomplishes a maximum thermoelectric figure of merit (ZT) of 0.86 near 480 K in x = 0.155. This is about 83 % more compared to that of bulk Ag2Te, and shows a significant improvement over the best value reported for Ag2Te nanostructures thus far. This study, therefore, shows that simultaneous nanocomposite formation, doping and nanostructuring could be an effective strategy for tuning the electron and phonon transports to improve the thermoelectric properties of a material.",2210.13903v1 2022-12-28,An Atomistic Model of Field-Induced Resistive Switching in Valence Change Memory,"In Valence Change Memory (VCM) cells, the conductance of an insulating switching layer is reversibly modulated by creating and redistributing point defects under an external field. Accurate simulations of the switching dynamics of these devices can be difficult due to their typically disordered atomic structures and inhomogeneous arrangements of defects. To address this, we introduce an atomistic framework for modelling VCM cells. It combines a stochastic Kinetic Monte Carlo approach for atomic rearrangement with a quantum transport scheme, both parameterized at the ab-initio level by using inputs from Density Functional Theory (DFT). Each of these steps operates directly on the underlying atomic structure. The model thus directly relates the energy landscape and electronic structure of the device to its switching characteristics. We apply this model to simulate non-volatile switching between high- and low-resistance states in an TiN/HfO2/Ti/TiN stack, and analyze both the kinetics and stochasticity of the conductance transitions. We also resolve the atomic nature of current flow resulting from the valence change mechanism, finding that conductive paths are formed between the undercoordinated Hf atoms neighboring oxygen vacancies. The model developed here can be applied to different material systems to evaluate their resistive switching potential, both for use as conventional memory cells and as neuromorphic computing primitives.",2212.14090v1 2023-05-02,Direct observations of spin fluctuations in spin-hedgehog-anti-hedgehog lattice states in MnSi$_{1-x}$Ge$_x$ ($x=0.6$ and $0.8$) at zero magnetic field,"The helimagnetic compounds MnSi$_{1-x}$Ge$_{x}$ show the three-dimensional multiple-$q$ order as referred to as spin-hedgehog-anti-hedgehog (SHAH) lattice. Two representative forms of SHAH are cubic-3$q$ lattice with $q \| \langle100\rangle$ and tetrahedral-4$q$ lattice with $q \| \langle111\rangle$, which show up typically for $x=1.0-~0.8$ and for $x=0.6$, respectively. Here, we have investigated the spin fluctuations in the MnSi$_{1-x}$Ge$_{x}$ polycrystalline samples with $x=0.6$ and $0.8$ by using the time-of-flight (TOF) neutron inelastic scattering and MIEZE-type neutron spin echo techniques to elucidate the microscopic origin of the unconventional Hall effect in the SHAH lattice states. This research is motivated by the observation of a sign change in the unconventional Hall resistivity as a function of temperature [Y. Fujishiro et al., Nat. Comm. $\textbf{10}$, 1059 (2019)]. The present results reveal the correspondences between the temperature ranges where the positive Hall resistivity and spin fluctuations are observed. These results agree well with the theoretical model of the conduction electrons scattered by the fluctuating spin clusters with a non-zero average of sign-biased scalar spin chirality as a mechanism of the positive Hall resistivity [H. Ishizuka and N. Nagaosa, Sci. Adv. $\textbf{4}$, eaap9962 (2018)].",2305.01172v1 2023-08-30,A Deep Dive into the Design Space of a Dynamically Reconfigurable Cryogenic Spiking Neuron,"Spiking neural network offers the most bio-realistic approach to mimic the parallelism and compactness of the human brain. A spiking neuron is the central component of an SNN which generates information-encoded spikes. We present a comprehensive design space analysis of the superconducting memristor (SM)-based electrically reconfigurable cryogenic neuron. A superconducting nanowire (SNW) connected in parallel with an SM function as a dual-frequency oscillator and two of these oscillators can be coupled to design a dynamically tunable spiking neuron. The same neuron topology was previously proposed where a fixed resistance was used in parallel with the SNW. Replacing the fixed resistance with the SM provides an additional tuning knob with four distinct combinations of SM resistances, which improves the reconfigurability by up to ~70%. Utilizing an external bias current (Ibias), the spike frequency can be modulated up to ~3.5 times. Two distinct spike amplitudes (~1V and ~1.8 V) are also achieved. Here, we perform a systematic sensitivity analysis and show that the reconfigurability can be further tuned by choosing a higher input current strength. By performing a 500-point Monte Carlo variation analysis, we find that the spike amplitude is more variation robust than spike frequency and the variation robustness can be further improved by choosing a higher Ibias. Our study provides valuable insights for further exploration of materials and circuit level modification of the neuron that will be useful for system-level incorporation of the neuron circuit",2308.15754v1 2023-12-03,Experimental apparatus for non-contact resistivity measurements of the rock core plug based on magnetic induction,"A new apparatus has been developed to measure the conductivity of rock samples. The probe, which consists of multi-coil transmitters and receivers doesn't require physical contact with the samples. The measurement is based on the induction principle. The measurement system is validated by using saline solutions and water-saturated sands of known conductivity. This work presents details of the development of a system of magnetic resistivity measurements by magnetic induction for petrophysical applications. The first application consists of measuring the resistivity of the core plug which is 0.038 m in diameter. Currently the system is operating properly at a frequency of 50 kHz with a current of up to 500 mA at 20 {\deg}C. During the study two types of samples were investigated: aqueous solutions with conductivities between 1 to 100 mS/cm and rocks. Several tests were carried out with the objective of investigating the performance of the instrument, such as the experiment to obtain sensitivity for the measurement system as a function of the current applied to the transmitter coil.",2312.01375v1 2023-12-08,The Kernel Method for Electrical Resistance Tomography,"In this paper we consider the inverse problem of electrical conductivity retrieval starting from boundary measurements, in the framework of Electrical Resistance Tomography (ERT). In particular, the focus is on non-iterative reconstruction algorithms, compatible with real-time applications. In this work a new non-iterative reconstruction method for Electrical Resistance Tomography, termed Kernel Method, is presented. The imaging algorithm deals with the problem of retrieving the shape of one or more anomalies embedded in a known background. The foundation of the proposed method is given by the idea that if there exists a current flux at the boundary (Neumann data) able to produce the same voltage measurements on two different configurations, with and without the anomaly, respectively, then the corresponding electric current density for the problem involving only the background material vanishes in the region occupied by the anomaly. Coherently with this observation, the Kernel Method consists in (i) evaluating a proper current flux at the boundary $g$, (ii) solving one direct problem on a configuration without anomaly and driven by $g$, (iii) reconstructing the anomaly from the spatial plot of the power density as the region in which the power density vanishes. This new tomographic method has a very simple numerical implementation at a very low computational cost. Beside theoretical results and justifications of our method, we present a large number of numerical examples to show the potential of this new algorithm.",2312.05059v1 2024-01-08,Microwave-assisted synthesis of LaMnO3+d: Tuning physical properties with microwave power,"Synthesis of transition metal oxides by microwave irradiation is a faster and energy-saving method compared to conventional heating in an electrical furnace because microwave energy is directly converted into heat within precursors. However, not much is known about how the physical properties are modified by the power of microwaves. We synthesized LaMnO3+d by irradiating oxide precursors with microwaves and studied the impact of microwave power (P = 1000 W, 1200 W, 1400 W and 1600 W) on magnetism, resistivity, magnetoresistance, thermopower, magnetic entropy change, magnetostriction, and electron spin resonance. It is found that paramagnetic to ferromagnetic transition becomes sharper, saturation magnetization increases, and electrical resistivity at low temperatures dramatically decreases as P increases. While the resistivity of samples irradiated with MW power of P less than or equal to 1400 W show insulating-like behavior down to 50 K, an insulator-metal transition occurs in the sample exposed to P = 1600 W and this sample also shows a maximum magnetoresistance (= -55%), magneto-thermopower (=-87%), magnetostriction (-180 x10-6) for H = 50 kOe and magnetic entropy change of 4.78 J/kg. K for H = 30 kOe around the Curie temperature. The intensity of electron spin resonance spectra at 300 K increases with P. We postulate that the much enhanced physical properties observed for the P = 1600 W sample arise from the creation of higher hole density, chemical homogeneity, and increased grain size. Our study shows that microwave power can be used as a knob to tune magnetism and other physical properties to our advantage.",2401.04087v1 2024-01-30,Two-Dimensional Phase-Fluctuating Superconductivity in Bulk-Crystalline NdO$_{0.5}$F$_{0.5}$BiS$_2$,"We present a combined growth and transport study of superconducting single-crystalline NdO$_{0.5}$F$_{0.5}$BiS$_2$. Evidence of two-dimensional superconductivity with significant phase fluctuations of preformed Cooper pairs preceding the superconducting transition is reported. This result is based on three key observations. (1) The resistive superconducting transition temperature $T_c$ (defined by resistivity $\rho \rightarrow 0$) increases with increasing disorder. (2) As $T\rightarrow T_c$, the conductivity diverges significantly faster than what is expected from Gaussian fluctuations in two and three dimensions. (3) Non-Ohmic resistance behavior is observed in the superconducting state. Altogether, our observations are consistent with a temperature regime of phase-fluctuating superconductivity. The crystal structure with magnetic ordering tendencies in the NdO$_{0.5}$F$_{0.5}$ layers and (super)conductivity in the BiS$_2$ layers is likely responsible for the two-dimensional phase fluctuations. As such, NdO$_{0.5}$F$_{0.5}$BiS$_2$ falls into the class of unconventional ``laminar"" bulk superconductors that include cuprate materials and 4Hb-TaS$_2$.",2401.16980v2 2024-02-11,Reducing the metal-graphene contact resistance through laser-induced defects,"Graphene has been extensively studied for a variety of electronic and optoelectronic applications. The reported contact resistance between metal and graphene, or rather its specific contact resistance (R{_C}), ranges from a few tens of {\Omega} {\mu}m up to a few k{\Omega} {\mu}m. Manufacturable solutions for defining ohmic contacts to graphene remain a subject of research. Here, we report a scalable method based on laser irradiation of graphene to reduce the R{_C} in nickel-contacted devices. A laser with a wavelength of {\lambda} = 532 nm is used to induce defects at the contact regions, which are monitored \textit{in-situ} using micro-Raman spectroscopy. Physical damage is observed using \textit{ex-situ} atomic force and scanning electron microscopy. The transfer line method (TLM) is used to extract R{_C} from back-gated graphene devices with and without laser treatment under ambient and vacuum conditions. A significant reduction in R{_C} is observed in devices where the contacts are laser irradiated, which scales with the laser power. The lowest R{_C} of about 250 {\Omega} {\mu}m is obtained for the devices irradiated with a laser power of 20 mW, compared to 900 {\Omega} {\mu}m for the untreated devices. The reduction is attributed to an increase in defect density, which leads to the formation of crystallite edges and in-plane dangling bonds that enhance the injection of charge carriers from the metal into the graphene. Our work suggests laser irradiation as a scalable technology for R{_C} reduction in graphene and potentially other two-dimensional materials.",2402.07151v1 2024-04-19,A Soft e-Textile Sensor for Enhanced Deep Learning-based Shape Sensing of Soft Continuum Robots,"The safety and accuracy of robotic navigation hold paramount importance, especially in the realm of soft continuum robotics, where the limitations of traditional rigid sensors become evident. Encoders, piezoresistive, and potentiometer sensors often fail to integrate well with the flexible nature of these robots, adding unwanted bulk and rigidity. To overcome these hurdles, our study presents a new approach to shape sensing in soft continuum robots through the use of soft e-textile resistive sensors. This sensor, designed to flawlessly integrate with the robot's structure, utilizes a resistive material that adjusts its resistance in response to the robot's movements and deformations. This adjustment facilitates the capture of multidimensional force measurements across the soft sensor layers. A deep Convolutional Neural Network (CNN) is employed to decode the sensor signals, enabling precise estimation of the robot's shape configuration based on the detailed data from the e-textile sensor. Our research investigates the efficacy of this e-textile sensor in determining the curvature parameters of soft continuum robots. The findings are encouraging, showing that the soft e-textile sensor not only matches but potentially exceeds the capabilities of traditional rigid sensors in terms of shape sensing and estimation. This advancement significantly boosts the safety and efficiency of robotic navigation systems.",2404.12627v1 1996-01-23,"Transport Properties, Thermodynamic Properties, and Electronic Structure of SrRuO3","SrRuO$_3$ is a metallic ferromagnet. Its electrical resistivity is reported for temperatures up to 1000K; its Hall coefficient for temperatures up to 300K; its specific heat for temperatures up to 230K. The energy bands have been calculated by self-consistent spin-density functional theory, which finds a ferromagnetic ordered moment of 1.45$\mu_{{\rm B}}$ per Ru atom. The measured linear specific heat coefficient $\gamma$ is 30mJ/mole, which exceeds the theoretical value by a factor of 3.7. A transport mean free path at room temperature of $\approx 10 \AA$ is found. The resistivity increases nearly linearly with temperature to 1000K in spite of such a short mean free path that resistivity saturation would be expected. The Hall coefficient is small and positive above the Curie temperature, and exhibits both a low-field and a high-field anomalous behavior below the Curie temperature.",9601106v1 1997-08-26,Scaling and the Metal-Insulator Transition in Si/SiGe Quantum Wells,"The existence of a metal-insulator transition at zero magnetic field in two- dimensional electron systems has recently been confirmed in high mobility Si-MOSFETs. In this work, the temperature dependence of the resistivity of gated Si/SiGe/Si quantum well structures has revealed a similar metal- insulator transition as a function of carrier density at zero magnetic field. We also report evidence for a Coulomb gap in the temperature dependence of the resistivity of the dilute 2D hole gas confined in a SiGe quantum well. In addition, the resistivity in the insulating phase scales with a single parameter, and is sample independent. These results are consistent with the occurrence of a metal-insulator transition at zero magnetic field in SiGe square quantum wells driven by strong hole-hole interactions.",9708201v1 1999-10-29,Neighbor-junction state effect on the fluxon motion in a Josephson stack,"We study experimentally and theoretically the influence of phase-whirling (resistive) state in one junction of a two-fold Josephson stack on the fluxon motion in the other junction. In experiment, we measure the fluxon velocity versus current in one junction as a function of the state (Meissner or resistive) of the neighboring junction. The analysis, made for the limit of high fluxon density, shows that the interaction with the resistive state results in an increase of the effective damping for the moving fluxon and, therefore, in reduction of its velocity. Numerical simulations confirm this result for various fluxon densities. The experimental data are in good agreement with the theoretical predictions. In addition, the fluxon step measured experimentally has a rather peculiar structure with back and forth bending regions which is understood as a manifestation of the photon absorption in the neighboring junction.",9910489v1 2000-03-02,Probing spin-charge separation using spin transport,"Pedagogical discussions are given on what constitutes a signature of spin-charge separation. A proposal is outlined to probe spin-charge separation in the normal state of the high $T_c$ cuprates using spin transport. Specifically, the proposal is to compare the temperature dependences of the spin resistivity and electrical resistivity: Spin-charge separation will be manifested in the different temperature dependences of these two resistivities. We also estimate the spin diffusion length and spin relaxation time scales, and we argue that it should be experimentally feasible to measure the spin transport properties in the cuprates using the spin-injection technique. The on-going spin-injection experiments in the cuprates and related theoretical issues are also discussed.",0003033v2 2000-06-01,Superconducting properties of [BaCuO_x]_2/[CaCuO_2]_n artificial structures with ultrathick CaCuO_2 blocks,"The electrical transport properties of [BaCuO_x]_2/[CaCuO_2]_n (CBCCO-2xn)underdoped high temperature superconducting superlattices grown by Pulsed Laser Deposition have been investigated. Starting from the optimally doped CBCCO-2x2 superlattice, having three CuO_2 planes and T_c around 80 K, we have systematically increased the number n up to 15 moving toward the underdoped region and hence decreasing T_c. For n>11 the artificial structures are no longer superconducting, as expected, for a uniformly distributed charge carriers density inside the conducting block layer. The sheet resistance of such artificial structures (n nearly equal to 11) turns out to be quite temperature independent and close to the 2D quantum resistance 26 kOhm. A further increase of the number of CuO_2 planes results in an insulator-type dependence of R(T) in the wide range of temperatures from room temperature to 1 K. The value of the sheet resistance separating the Superconducting and the Insulating regimes supports the fermionic scenario of the Superconductor-Insulator transition in these systems.",0006023v2 2000-08-02,Evidence for small or intermediate-size polarons in the ferromagnetic state of manganites,"Oxygen-isotope effects on the intrinsic resistivity have been studied in high-quality epitaxial thin films of La_{0.75}Ca_{0.25}MnO_{3} and Nd_{0.7}Sr_{0.3}MnO_{3}. We found that the residual resistivity \rho_{o} increases by about 15(3)% upon replacing ^{16}O by ^{18}O. This provides strong evidence for the presence of small or intermediate-size polarons in the metallic ferromagnetic state. Furthermore, the temperature dependent part of the resistivity at low temperatures consists of an AT^{4.5} term contributed from 2-magnon scattering, and a B\omega_{s}/\sinh^{2}(\hbar\omega_{s}/2k_{B}T) term which arises from scattering by a soft optical phonon mode. The absolute magnitudes of the coefficient A and the phonon frequency \hbar\omega_{s} for both isotope samples are in quantitative agreement with theoretical predictions.",0008029v1 2000-10-06,Fluctuation Effects in High Sheet Resistance Superconducting Films,"As the normal state sheet resistance, $R_n$, of a thin film superconductor increases, its superconducting properties degrade. For $R_n\simeq h/4e^2$ superconductivity disappears and a transition to a nonsuperconducting state occurs. We present electron tunneling and transport measurements on ultrathin, homogeneously disordered superconducting films in the vicinity of this transition. The data provide strong evidence that fluctuations in the amplitude of the superconducting order parameter dominate the tunneling density of states and the resistive transitions in this regime. We briefly discuss possible sources of these amplitude fluctuation effects. We also describe how the data suggest a novel picture of the superconductor to nonsuperconductor transition in homogeneous 2D systems.",0010114v1 2001-07-29,Pressure-induced Superconductivity in a Ferromagnet UGe$_2$ -- Resistivity Measurements in Magnetic Field --,"The electrical resistivity measurements in the magnetic field are carried out on the pressure-induced superconductor UGe$_2$. The superconductivity is observed from 1.06 to 1.44 GPa. The upper critical field of $H_{C2}$ is anisotropic where $H_{C2}(T)$ exhibits positive curvature for $H//b$ and $c$-axis. The characteristic enhancement of $H_{C2}$ is reconfirmed for $H//a$-axis. In the temperature and field dependence of resistivity at $P > P_{C}$ where the ferromagnetic ordering disappears, it is observed that the application of the external field along the {\it a}-axis increases the coefficient of Fermi liquid behavior $AT^{2}$ correspondingly to the metamagnetic transition.",0107584v1 2001-10-26,Two-dimensional metal in a parallel magnetic field,"We have investigated the effect of an in plane parallel magnetic field (B_||) on two high mobility metallic-like dilute two-dimensional hole gas (2DHG) systems in GaAs quantum wells. The experiments reveal that, while suppressing the magnitude of the low temperature resistance drop, B_|| does not affect E_a, the characteristic energy scale of the metallic resistance drop. The field B_c at which the metallic-like resistance drop vanishes is dependent on both the width of quantum well and the orientation of B_||. It is unexpected that E_a is unaffected by B_|| up to Bc depite that the Zeeman energy at B_c is roughly equal to E_a.",0110571v1 2002-05-07,Doping Dependence of Anisotropic Resistivities in Trilayered Superconductor Bi2Sr2Ca2Cu3O10+delta (Bi-2223),"The doping dependence of the themopower, in-plane resistivity rho_ab(T), out-of-plane resistivity rho_c(T), and susceptibility has been systematically measured for high-quality single crystal Bi2Sr2Ca2Cu3O10+delta. We found that the transition temperature Tc and pseudogap formation temperature T_rho_c*, below which rho_c shows a typical upturn, do not change from their optimum values in the ""overdoped"" region, even though doping actually proceeds. This suggests that, in overdoped region, the bulk $T_c$ is determined by the always underdoped inner plane, which have a large superconducting gap, while the carriers are mostly doped in the outer planes, which have a large phase stiffness.",0205121v1 2002-09-19,Temperature dependence of electrical resistivity of high-Tc cuprates - from pseudogap to overdoped regions,"The effects of planar hole concentration, p, and in-plane disorder, Zn (y), on the DC resistivity, r(T), of sintered samples of Y_{1-x}Ca_xBa_2(Cu_{1-y}Zn_y)_3O_{7-d} were investigated over a wide doping range by changing both the oxygen deficiency (d) and Ca content (x). From the r(T,p) data we extracted characteristic crossover temperatures on the underdoped and overdoped sides, T* and T_m respectively, above which r(T) is linear. We compare our results with a number of other polycrystalline, thin film and single crystal cuprate superconductors and find similar behavior in the p-dependence of T*(p), T_m(p), and the resistivity exponent, m(p), in fits to r(T) = r_0 + aT^m on the overdoped side. Our findings point towards the possible existence of a quantum critical point (QCP) at the doping p=0.19 +/- 0.01.",0209457v1 2002-10-23,Crossover from coherent to incoherent electronic excitations in the normal state of Bi2Sr2CaCu2O8,"Angle resolved photoemission spectroscopy (ARPES) and resistivity measurements are used to explore the overdoped region of the high temperature superconductor Bi2Sr2CaCu2O8+delta. We find evidence for a new crossover line in the phase diagram between a coherent metal phase for lower temperatures and higher doping, and an incoherent metal phase for higher temperatures and lower doping. The former is characterized by two well-defined spectral peaks in ARPES due to coherent bilayer splitting and superlinear behavior in the resistivity, whereas the latter is characterized by a single broad spectral feature in ARPES and a linear temperature dependence of the resistivity.",0210531v1 2003-01-14,Resistance Noise Scaling in a Dilute Two-Dimensional Hole System in GaAs,"We have measured the resistance noise of a two-dimensional (2D)hole system in a high mobility GaAs quantum well, around the 2D metal-insulator transition (MIT) at zero magnetic field. The normalized noise power $S_R/R^2$ increases strongly when the hole density p_s is decreased, increases slightly with temperature (T) at the largest densities, and decreases strongly with T at low p_s. The noise scales with the resistance, $S_R/R^2 \sim R^{2.4}$, as for a second order phase transition such as a percolation transition. The p_s dependence of the conductivity is consistent with a critical behavior for such a transition, near a density p* which is lower than the observed MIT critical density p_c.",0301222v2 2003-01-29,Radiation-Induced Magnetoresistance Oscillations in a 2D Electron Gas,"Recent measurements of a 2D electron gas subjected to microwave radiation reveal a magnetoresistance with an oscillatory dependence on the ratio of radiation frequency to cyclotron frequency. We perform a diagrammatic calculation and find radiation-induced resistivity oscillations with the correct period and phase. Results are explained via a simple picture of current induced by photo-excited disorder-scattered electrons. The oscillations increase with radiation intensity, easily exceeding the dark resistivity and resulting in negative-resistivity minima. At high intensity, we identify additional features, likely due to multi-photon processes, which have yet to be observed experimentally.",0301569v3 2003-02-05,"A low density finite temperature apparent ""insulating"" phase in 2D systems","We propose that the observed low density ``insulating'' phase of a 2D semiconductor system, with the carrier density being just below ($n < n_c$) the so-called critical density where the derivative of resistivity changes sign at low temperatures (i.e. resistivity $\rho(T)$ increases with increasing $T$ for $n > n_c$ whereas it decreases with increasing $T$ for $n < n_c$), is in fact a ``high-temperature'' crossover version of the same effective metallic phase seen at higher densities ($n>n_c$). This low density ($nTm), the Rxy(T) dependence can be qualitatively explained in terms of either a semiclassical T-dependence of a transport time, or a thermal activation of carries from a localized band.",0504475v1 2005-06-12,Classical Hall transition and magnetoresistance in strongly inhomogeneous planar systems,"The magneto-transport properties of planar and layered strongly inhomogeneous two-phase systems are investigated, using the explicit expressions for the effective conductivities and resistivities obtained by the exact dual transformation, connecting effective conductivities of in-plane isotropic two-phase systems with and without magnetic field. These expressions allow to describe the effective resistivity of various inhomogeneous media at arbitrary concentrations $x$ and magnetic fields $H$. The corresponding plots of the $x$-dependence of the Hall constant $R_H(x,H)$ and the magnetoresistance $R(x,H)$ are constructed for various values of magnetic field at some values of inhomogeneity parameters. These plots for strongly inhomogeneous systems at high magnetic fields show a sharp transition between partial Hall resistivities (or Hall conductivities) with different dependencies of $R_H$ on the phase concentrations. It is shown that there is a strong correlation between large linear magnetoresistance effect and this sharp Hall transition. Both these effects are a consequence of the exact duality symmetry. A possible physical explanation of these effects and their correlation is proposed.",0506267v1 2005-07-08,Field-induced non-Fermi-liquid resistivity of stoichiometric YbAgGe single crystals,"We have investigated hexagonal YbAgGe down to 70 mK by measuring the magnetic-field and temperature dependence of the resistivity rho of single crystals in fields up to 14 T. Our results extend the H-T phase diagram to the lowest temperatures for H applied in the basal plane and along the c-axis. In particular, critical fields for the suppression of several magnetic phases are determined. The temperature dependence of rho(T) is unusual: whereas at low H, rho(T) reveals a temperature exponent n>=2, we find 1<=n<1.5 and strong enhancement of the temperature dependence of rho(T) close to and beyond the highest critical field for each field direction. For H applied in the basal plane, at high fields a conventional T^2 dependence of rho(T) is reached above 10 T accompanied by an approach to saturation of a strong drop in the residual resistivity. YbAgGe appears to be one of few Yb-based stoichiometric systems, where quantum-critical behaviour may be induced by a magnetic field.",0507211v2 2005-08-12,The microwave induced resistance response of a high mobility 2DEG from the quasi-classical limit to the quantum Hall regime,"Microwave induced resistance oscillations (MIROs) were studied experimentally over a very wide range of frequencies ranging from ~20 GHz up to ~4 THz, and from the quasi-classical regime to the quantum Hall effect regime. At low frequencies regular MIROs were observed, with a periodicity determined by the ratio of the microwave to cyclotron frequencies. For frequencies below 150 GHz the magnetic field dependence of MIROs waveform is well described by a simplified version of an existing theoretical model, where the damping is controlled by the width of the Landau levels. In the THz frequency range MIROs vanish and only pronounced resistance changes are observed at the cyclotron resonance. The evolution of MIROs with frequency are presented and discussed.",0508327v1 2005-11-15,1/f noise in a dilute GaAs two-dimensional hole system in the insulating phase,"We have measured the resistance and the 1/f resistance noise of a two-dimensional low density hole system in a high mobility GaAs quantum well at low temperature. At densities lower than the metal-insulator transition one, the temperature dependence of the resistance is either power-like or simply activated. The noise decreases when the temperature or the density increase. These results contradict the standard description of independent particles in the strong localization regime. On the contrary, they agree with the percolation picture suggested by higher density results. The physical nature of the system could be a mixture of a conducting and an insulating phase. We compare our results with those of composite thin films.",0511375v1 2006-02-03,Observation of the quantized Hall insulator in the quantum critical regime of the two-dimensional electron gas,"We have investigated the Hall resistance $R_H$ near the plateau-insulator transition of a two-dimensional electron gas in the quantum critical regime. High-field magnetotransport data taken on a low-mobility InGaAs/InP heterostructure with the plateau-insulator transition at a critical field $B_c$ of 17.2 T show that the Hall resistance $R_H$ is quantized at $h/e^2$ near the critical filling fraction ($\nu_c$ = 0.55) when $T \to 0$. By making use of universal scaling functions extracted from the magnetotransport data we show that $R_H$ in the insulating phase in the limit $T \to 0$ is quantized at $h/e^2$ for all values of the scaling parameter $\Delta\nu /(T/T_0)^\kappa$ with $\Delta\nu = \nu - \nu_c$. However, as a function of $\Delta\nu $ (or magnetic field) the Hall resistance diverges in the limit $T \to 0$ for all values $\nu < \nu_c$.",0602093v2 2006-12-18,Nonlinear Current of Strongly Irradiated Quantum Hall Gas,"Two dimensional electrons in weakly disordered high Landau levels are considered. The current-field response in the presence of a strong microwave field, is computed. The disordered Floquet evolution operator allows us to treat the short range disorder perturbatively, at any strength of electric fields. A simplifying Random Matrix Approximation reproduces the broadened Landau levels density of states and structure factor. We derive the magnitude of the Microwave Induced Resistivity Oscillations. The disorder short wavelength cut-off determines the non-linear electric fields of the Zero Resistance State and the Hall Induced Resistivity Oscillations. We discuss wider implications of our results on experiments and other theories.",0612469v2 2007-12-13,Study of GEM-like detectors with resistive electrodes for RICH applications,"We have developed prototypes of GEM-like detectors with resistive electrodes to be used as RICH photodetectors equipped with CsI photocathodes. The main advantages of these detectors are their intrinsic spark protection and possibility to operate at high gain (~10E5) in many gases including poorly quenched ones, allowing for the adoption of windowless configurations in which the radiator gas is also used in the chamber. Results of systematic studies of the resistive GEMs combined with CsI photocathodes are presented: its quantum efficiency, rate characteristics, long-term stability, etc. On the basis of the obtained results, we believe that the new detector will be a promising candidate for upgrading the ALICE RICH detector",0712.2179v1 2008-01-06,Scaling of Hall Resistivity in the Mixed State of MgB2 Films,"The longitudinal resistivity (rho_{xx}) and transverse resistivity (rho_{xy}) of MgB2 thin films in the mixed state were studied in detail. We found that the temperature dependencies of rho_{xx} and \rho_{xy} at a fixed magnetic field (H) satisfy the scaling law of $\rho_{xy}=A\rho_{xx}^\beta$, where the exponent beta varies around 2.0 for different fields. In the low field region (below 1T), beta maintains a constant value of 2.0 due to the weak pinning strength of the vortices, mainly from the superfluid of the pi band. When H>1T, beta drops abruptly to its lowest value at about 2T because of the proliferation of quasiparticles from the pi-band and, hence, the motion of the vortices from the superfluid of the sigma-band dominates the dissipation. As the field is increased further, the vortex pinning strength is weakened and beta increases monotonically towards 2.0 at a high field. All the results presented here are in good agreement with the expectation of the vortex physics of a multi-band superconductor.",0801.0838v1 2008-02-05,Effect of small particles on the near-wall dynamics of a large particle in a highly bidisperse colloidal solution,"We consider the hydrodynamic effect of small particles on the dynamics of a much larger particle moving normal to a planar wall in a highly bidisperse dilute colloidal suspension of spheres. The gap $h_0$ between the large particle and the wall is assumed to be comparable to the diameter $2a$ of the smaller particles so there is a length-scale separation between the gap width $h_0$ and the radius of the large particle $b< 0 properties suggest a new class of non-Fermi liquid.",0811.3439v1 2009-02-25,Resistive relaxation of a magnetically confined mountain on an accreting neutron star,"Three-dimensional numerical magnetohydrodynamic (MHD) simulations are performed to investigate how a magnetically confined mountain on an accreting neutron star relaxes resistively. No evidence is found for non-ideal MHD instabilities on a short time-scale, such as the resistive ballooning mode or the tearing mode. Instead, the mountain relaxes gradually as matter is transported across magnetic surfaces on the diffusion time-scale, which evaluates to $\tau_\mathrm{I} \sim 10^5 - 10^8$ yr (depending on the conductivity of the neutron star crust) for an accreted mass of $M_a = 1.2 \times 10^{-4} M_\odot$. The magnetic dipole moment simultaneously reemerges as the screening currents dissipate over $\tau_\mathrm{I}$. For nonaxisymmetric mountains, ohmic dissipation tends to restore axisymmetry by magnetic reconnection at a filamentary neutral sheet in the equatorial plane. Ideal-MHD oscillations on the Alfv\'{e}n time-scale, which can be excited by external influences, such as variations in the accretion torque, compress the magnetic field and hence decrease $\tau_\mathrm{I}$ by \change{one order of magnitude} relative to its standard value (as computed for the static configuration). The implications of long-lived mountains for gravitational wave emission from low-mass X-ray binaries are briefly explored.",0902.4484v1 2009-12-09,Coulomb zero bias anomaly for fractal geometry and conductivity of granular systems near the percolation threshold,"A granular system slightly below the percolation threshold is a collection of finite metallic clusters, characterized by wide spectrum of sizes, resistances, and charging energies. Electrons hop from cluster to clusters via short insulating ""links"" of high resistance. At low temperatures all clusters are Coulomb blockaded and the dc-conductivity is exponentially suppressed. At lowest T the leading transport mechanism is variable range cotunneling via largest (critical) clusters, leading to the modified Efros-Shklovsky law. At intermediate temperatures the principal suppression of the conductivity originates from the Coulomb zero bias anomaly occurring, when electron tunnels between adjacent large clusters with large resistances. Such clusters are essentially extended objects and their internal dynamics should be taken into account. In this regime the T-dependence of conductivity is stretched exponential with a nontrivial index, expressed through the indices of percolation theory. Due to the fractal structure of large clusters the anomaly is strongly enhanced: it arises not only in low dimensions, but also in d=3 case.",0912.1701v1 2010-02-16,Pseudogap Phase Boundary in Overdoped Bi_2Sr_2CaCu_2O_8 Studied by Measuring Out-of-plane Resistivity under the Magnetic Fields,"The characteristic pseudogap temperature T* in Bi2Sr2CaCu2O8 system has been systematically evaluated as a function of doping, especially focusing on its overdoped region, by measuring the out-of-plane resistivity under the magnetic fields. Overdoped samples have been prepared by annealing TSFZ-grown Bi2Sr2CaCu2O8 single crystals under the high oxygen pressures (990 kgf/cm2). At a zero field, the out-of-plane resistivity showed a metallic behavior down to Tc (= 62 K), while under the magnetic fields of over 3 T,it showed typical upturn behavior from around 65 K upon decreasing temperature. This result suggests that the pseudogap and superconductivity are different phenomena.",1002.3014v1 2010-05-13,Probing top-gated field effect transistor of reduced graphene oxide monolayer made by dielectrophoresis,"We demonstrate top-gated field effect transistor made of reduced graphene oxide (RGO) monolayer (graphene) by dielectrophoresis. Raman spectrum of RGO flakes of typical size of 5{\mu}m x 5{\mu}m show a single 2D band at 2687 cm-1, characteristic of a single layer graphene. The two probe current - voltage measurements of RGO flakes, deposited in between the patterned electrodes with a gap of 2.5 {\mu}m using a.c. dielectrophoresis show ohmic behavior with a resistance of ~ 37k{\Omega}. The temperature dependence of the resistance (R) of RGO measured between temperatures 305 K to 393 K yields temperature coefficient of resistance [dR/dT]/R ~ -9.5x10-4 K-1, same as mechanically exfoliated single layer graphene. The field effect transistor action was obtained by electrochemical top-gating using solid polymer electrolyte (PEO + LiClO4) and Pt wire. Ambipolar nature of graphene flakes is observed upto a doping level of ~ 6x1012/cm2 and carrier mobility of ~ 50 cm2V-1sec-1. The source - drain current characteristics shows a tendency of current saturation at high source - drain voltage which is analyzed quantitatively by a diffusive transport model.",1005.2258v1 2010-08-10,Temperature-dependent resistivity of suspended graphene,"In this paper we investigate the electron-phonon contribution to the resistivity of suspended single layer graphene. In-plane as well as flexural phonons are addressed in different temperature regimes. We focus on the intrinsic electron-phonon coupling due to the interaction of electrons with elastic deformations in the graphene membrane. The competition between screened deformation potential vs fictitious gauge field coupling is discussed, together with the role of tension in the suspended flake. In the absence of tension, flexural phonons dominate the phonon contribution to the resistivity at any temperature $T$ with a $T^{5/2}_{}$ and $T^{2}_{}$ dependence at low and high temperatures, respectively. Sample-specific tension suppresses the contribution due to flexural phonons, yielding a linear temperature dependence due to in-plane modes. We compare our results with recent experiments.",1008.1631v1 2010-08-17,Heat capacity study of BaFe$_{2}$As$_{2}$: effects of annealing,"Heat-capacity, X-ray diffraction, and resistivity measurements on a high-quality BaFe$_{2}$As$_{2}$ sample show an evolution of the magneto-structural transition with successive annealing periods. After a 30-day anneal the resistivity in the (ab) plane decreases by more than an order of magnitude, to 12 $\mu\Omega$cm, with a residual resistance ratio $\sim$36; the heat-capacity anomaly at the transition sharpens, to an overall width of less than K, and shifts from 135.4 to 140.2 K. The heat-capacity anomaly in both the as-grown sample and after the 30-day anneal shows a hysteresis of $\sim$0.15 K, and is unchanged in a magnetic field $\mu_{0}$H = 14 T. The X-ray and heat-capacity data combined suggest that there is a first order jump in the structural order parameter. The entropy of the transition is reported.",1008.2967v2 2010-09-17,Anomalously strong pinning of the filling factor nu=2 in epitaxial graphene,"We explore the robust quantization of the Hall resistance in epitaxial graphene grown on Si-terminated SiC. Uniquely to this system, the dominance of quantum over classical capacitance in the charge transfer between the substrate and graphene is such that Landau levels (in particular, the one at exactly zero energy) remain completely filled over an extraordinarily broad range of magnetic fields. One important implication of this pinning of the filling factor is that the system can sustain a very high nondissipative current. This makes epitaxial graphene ideally suited for quantum resistance metrology, and we have achieved a precision of 3 parts in 10^10 in the Hall resistance quantization measurements.",1009.3450v3 2010-10-14,Resistivity and Hall effect of LiFeAs: Evidence for electron-electron scattering,"LiFeAs is unique among the broad family of FeAs-based superconductors, because it is superconducting with a rather large $T_c\simeq 18$ K under ambient conditions although it is a stoichiometric compound. We studied the electrical transport on a high-quality single crystal. The resistivity shows quadratic temperature dependence at low temperature giving evidence for strong electron-electron scattering and a tendency towards saturation around room temperature. The Hall constant is negative and changes with temperature, what most probably arises from a van Hove singularity close to the Fermi energy in one of the hole-like bands. Using band structure calculations based on angular resolved photoemission spectra we are able to reproduce all the basic features of both the resistivity as well as the Hall effect data.",1010.2876v2 2010-10-20,Raychaudhuri's equation and aspects of relativistic charged collapse,"We use the Raychaudhuri equation to probe certain aspects related to the gravitational collapse of a charged medium. The aim is to identify the stresses the Maxwell field exerts on the fluid and discuss their potential implications. Particular attention is given to those stresses that resist contraction. After looking at the general case, we consider the two opposite limits of poor and high electrical conductivity. In the former there are electric fields but no currents, while in the latter the situation is reversed. When the conductivity is low, we find that the main agents acting against the collapse are the Coulomb forces triggered by the presence of an excess charge. At the ideal Magnetohydrodynamic (MHD) limit, on the other hand, the strongest resistance seems to come from the tension of the magnetic forcelines. In either case, we discuss whether and how the aforementioned resisting stresses may halt the contraction and provide a set of conditions making this likely to happen.",1010.4211v2 2010-12-30,Pressure-Driven Quantum Criticality in An Iron-Selenide Superconductor,"The discovery of superconductivity of about 30 K in iron selenides with very large magnetic moments simulates the examination of completing orders. Here we report a finding of pressure- induced suppression of the superconducting transition temperature Tc and enhancement of the temperature of the resistance hump TH through charge transfer between two iron sites with different occupancies. The activation energy for the electric transport of the high-temperature resistance is observed to go to zero at a critical pressure of 8.7 GPa, at which superconductivity tends to disappear and the semiconductor-to-metal transition takes place. Beyond the critical point, the resistance exhibits a metallic behavior over the whole temperature range studied. All these features indicate the existence of quantum criticality in iron-selenide superconductors.",1101.0092v3 2011-02-22,Charged Dilatonic Black Holes and their Transport Properties,"We briefly explain the consistency conditions imposed on the effective holographic theories, which are parameterized by two real exponents $(\gamma,\delta)$ that control the IR dynamics. The general scaling of DC resistivity with temperature at low temperature and AC conductivity at low frequency across the whole $(\gamma,\delta)$ plane are explained. There is a codimension-one region where the DC resistivity is linear in the temperature. For massive carriers, it is shown that when the scalar operator is not the dilaton, the DC resistivity scales as the heat capacity (and entropy) for $(2+1)$-dimensional systems. Regions are identified where the theory at finite density is a Mott-like insulator. This contribution is based on arXiv:1005.4690 with emphasis on the transport properties of charged dilatonic black holes with potential.",1102.4440v1 2011-03-24,Collective excitations and low temperature transport properties of bismuth,"We examine the influence of collective excitations on the transport properties (resistivity, magneto- optical conductivity) for semimetals, focusing on the case of bismuth. We show, using an RPA approximation, that the properties of the system are drastically affected by the presence of an acoustic plasmon mode, consequence of the presence of two types of carriers (electrons and holes) in this system. We found a crossover temperature T* separating two different regimes of transport. At high temperatures T > T* we show that Baber scattering explains quantitatively the DC resistivity experiments, while at low temperatures T < T* interactions of the carriers with this collective mode lead to a T^5 behavior of the resistivity. We examine other consequences of the presence of this mode, and in particular predict a two plasmon edge feature in the magneto-optical conductivity. We compare our results with the experimental findings on bismuth. We discuss the limitations and extensions of our results beyond the RPA approximation, and examine the case of other semimetals such as graphite or 1T-TiSe_2.",1103.4850v1 2011-03-29,Substrate Gating of Contact Resistance in Graphene Transistors,"Metal contacts have been identified to be a key technological bottleneck for the realization of viable graphene electronics. Recently, it was observed that for structures that possess both a top and a bottom gate, the electron-hole conductance asymmetry can be modulated by the bottom gate. In this letter, we explain this observation by postulating the presence of an effective thin interfacial dielectric layer between the metal contact and the underlying graphene. Electrical results from quantum transport calculations accounting for this modified electrostatics corroborate well with the experimentally measured contact resistances. Our study indicates that the engineering of metal- graphene interface is a crucial step towards reducing the contact resistance for high performance graphene transistors.",1103.5773v2 2011-05-28,A New numerical scheme for resistive relativistic MHD using method of characteristics,"We present a new numerical method of special relativistic resistive magnetohydrodynamics with scalar resistivity that can treat a range of phenomena, from nonrelativistic to relativistic (shock, contact discontinuity, and Alfv\'en wave). The present scheme calculates the numerical flux of fluid by using an approximate Riemann solver, and electromagnetic field by using the method of characteristics. Since this scheme uses appropriate characteristic velocities, it is capable of accurately solving problems that cannot be approximated as ideal magnetohydrodynamics and whose characteristic velocity is much lower than light velocity. The numerical results show that our scheme can solve the above problems as well as nearly ideal MHD problems. Our new scheme is particularly well suited to systems with initially weak magnetic field, and mixed phenomena of relativistic and non-relativistic velocity; for example, MRI in accretion disk, and super Alfv\'enic turbulence.",1105.5683v1 2011-06-02,High Lundquist Number Resistive MHD Simulations of Magnetic Reconnection: Searching for Secondary Island Formation,"Recently, secondary island formation due to the tearing instability of the Sweet-Parker current sheet was identified as a possible mechanism that can lead to fast reconnection (less sensitive dependence on Lundquist number $S$) both in numerical simulations using Particle-in-Cell (PIC) method [Daughton et al. 2009], as well as using resistive magnetohydrodynamics (MHD) [Lapenta 2008; Bhattacharjee et al. 2009]. This instability is thought to appear when $S$ is greater than a certain threshold. These recent results prompt us to perform more resistive MHD simulations of a basic reconnection configuration based on the island coalescence instability, using much higher resolutions and larger $S$. Our simulations are based on a fairly standard pseudo spectral code, which has been tested for accuracy, convergence, and compared well with codes using other methods [Ng et al. 2008]. In our simulations, formation of plasmoids were not found, except when insufficient resolution was used, or when a small amount of noise was added externally. The reconnection rate is found to follow the Sweet-Parker scaling when no noise is added, but increases to a level independent of $S$ with noise, when plasmoids form. Latest results with $S$ up to $2 \times 10^5$ will be presented.",1106.0521v1 2011-08-03,Unusual Field-Insensitive Phase Transition and Kondo Behavior in SmTi$_2$Al$_{20}$,"Magnetization, electrical resistivity and specific heat measurements were performed on high-quality single crystalline SmTi$_2$Al$_{20}$ (residual resistivity ratio $\sim$ 40) grown by Al self-flux method. A Kondo-like $\log T$ dependence in the resistivity is observed below 50 K. We discovered a field-insensitive phase transition at $T_{x}$ = 6.5 K and a field-insensitive heavy fermion behavior with the electronic specific heat coefficient $\gamma$ = 150 mJ/(K$^{2}$ mol). Specific heat analysis reveals that the ground state is a $\Gamma_{8}$ quartet state and the Sm magnetic dipole moment $m_{{\rm Sm}}$ ($\sim 0.5 \mu_{{\rm B}}$ at $T \simeq$ 0) orders below $T_{x}$ in spite of the field-insensitive behavior. Possible reasons for the field insensitiveness will be discussed.",1108.0751v1 2011-08-15,Current-Controlled Negative Differential Resistance due to Joule Heating in TiO2,"We show that Joule heating causes current-controlled negative differential resistance (CC-NDR) in TiO2 by constructing an analytical model of the voltage-current V(I) characteristic based on polaronic transport for Ohm's Law and Newton's Law of Cooling, and fitting this model to experimental data. This threshold switching is the 'soft breakdown' observed during electroforming of TiO2 and other transition-metal-oxide based memristors, as well as a precursor to 'ON' or 'SET' switching of unipolar memristors from their high to their low resistance states. The shape of the V(I) curve is a sensitive indicator of the nature of the polaronic conduction.",1108.3120v1 2011-08-25,Generalized four-point characterization method for resistive and capacitive contacts,"In this paper, a four-point characterization method is developed for resistive samples connected to either resistive or capacitive contacts. Provided the circuit equivalent of the complete measurement system is known including coaxial cable and connector capacitances as well as source output and amplifier input impedances, a frequency range and capacitive scaling factor can be determined, whereby four-point characterization can be performed. The technique is demonstrated with a discrete element test sample over a wide frequency range using lock-in measurement techniques from 1 Hz - 100 kHz. The data fit well with a circuit simulation of the entire measurement system. A high impedance preamplifier input stage gives best results, since lock-in input impedances may differ from manufacturer specifications. The analysis presented here establishes the utility of capacitive contacts for four-point characterizations at low frequency.",1108.5006v1 2011-09-09,Details of Sample Dependence and Transport Properties of URu2Si2,"Resistivity and specific heat measurements were performed in the low carrier unconventional superconductor URu2Si2 on various samples with very different qualities. The superconducting transition temperature (TSC) and the hidden order transition temperature (THO) of these crystals were evaluated as a function of the residual resistivity ratio (RRR). In high quality single crystals the resistivity does not seem to follow a T2 dependence above TSC, indicating that the Fermi liquid regime is restricted to low temperatures. However, an analysis of the isothermal longitudinal magnetoresistivity points out that the T2 dependence may be ""spoiled"" by residual inhomogeneous superconducting contribution. We discuss a possible scenario concerning the distribution of TSC related with the fact that the hidden order phase is very sensitive to the pressure inhomogeneity.",1109.1953v1 2011-11-15,Phenomenology of retained refractoriness: On semi-memristive discrete media,"We study two-dimensional cellular automata, each cell takes three states: resting, excited and refractory. A resting cell excites if number of excited neighbours lies in a certain interval (excitation interval). An excited cell become refractory independently on states of its neighbours. A refractory cell returns to a resting state only if the number of excited neighbours belong to recovery interval. The model is an excitable cellular automaton abstraction of a spatially extended semi-memristive medium where a cell's resting state symbolises low-resistance and refractory state high-resistance. The medium is semi-memristive because only transition from high- to low-resistance is controlled by density of local excitation. We present phenomenological classification of the automata behaviour for all possible excitation intervals and recovery intervals. We describe eleven classes of cellular automata with retained refractoriness based on criteria of space-filling ratio, morphological and generative diversity, and types of travelling localisations.",1111.3525v1 2011-12-06,Homogeneous bilayer graphene film based flexible transparent conductor,"Graphene is considered a promising candidate to replace conventional transparent conductors due to its low opacity, high carrier mobility and flexible structure. Multi-layer graphene or stacked single layer graphenes have been investigated in the past but both have their drawbacks. The uniformity of multi-layer graphene is still questionable, and single layer graphene stacks require many transfer processes to achieve sufficiently low sheet resistance. In this work, bilayer graphene film grown with low pressure chemical vapor deposition was used as a transparent conductor for the first time. The technique was demonstrated to be highly efficient in fabricating a conductive and uniform transparent conductor compared to multi-layer or single layer graphene. Four transfers of bilayer graphene yielded a transparent conducting film with a sheet resistance of 180 {\Omega}_{\square} at a transmittance of 83%. In addition, bilayer graphene films transferred onto plastic substrate showed remarkable robustness against bending, with sheet resistance change less than 15% at 2.14% strain, a 20-fold improvement over commercial indium oxide films.",1112.1378v1 2012-04-12,Nonequilibrium quasiparticles and electron cooling by normal metal - superconductor tunnel junctions,"We consider a model NISIN system with two junctions in series, where N is a normal metal, S is a superconductor and I is an insulator. We assume that the resistance of the first junction is high, while the resistance of the second one is low. In this case the first junction cools the left normal electrode, while the second junction partially removes excited quasiparticles from the superconductor. We consider cooling properties of this double junction structure. It is shown that the cooling power depends strongly on the ratio of the resistances of the two junctions. In conclusion, we derive a generalized expression for the cooling power of a NIS tunnel junction taking into account charge imbalance effects.",1204.2719v1 2012-05-31,High-pressure study of non-Fermi liquid and spin-glass-like behavior in CeRhSn,"We present measurements of the temperature dependence of electrical resistivity of CeRhSn up to ~ 27 kbar. At low temperatures, the electrical resistivity varies linearly with temperature for all pressures, indicating non-Fermi liquid behavior. Below a temperature Tf ~ 6 K, the electrical resistivity deviates from a linear dependence. We found that the low-temperature feature centered at T = Tf shows a pressure dependence dTf/dP ~ 30 mK/kbar which is typical of canonical spin glasses. This interplay between spin-glass-like and non-Fermi liquid behavior was observed in both CeRhSn and a Ce0.9La0.1RhSn alloy.",1205.6997v1 2012-07-13,Effect of boron doping in the microwave surface resistance of neutron irradiated melt-textured Y_1.6Ba_2.3Cu_3.3O_7-x samples,"We report on the microwave surface resistance of melt-textured Y_1.6Ba_2.3Cu_3.3O_7-x samples, doped with different amount of B_2O_3 and, subsequently, irradiated by thermal neutrons at the fluence of 1.476 \times 10^17 cm^-2. The microwave surface resistance has been measured as a function of temperature and DC magnetic field. The experimental results are quantitatively discussed in the framework of the Coffey and Clem theory, properly adapted to take into account the d-wave nature of cuprate superconductors. By fitting the experimental data at zero DC field, we have highlighted the effects of the induced defects in the general properties of the samples, including the intergranular region. The analysis of the results obtained at high DC fields allowed us to investigate the fluxon dynamics and deduce the depinning frequency; in particular, we have shown that the addition of B_2O_3 up to 0.1 wt% increases the effectiveness of the defects to hinder the fluxon motion induced by the microwave current.",1207.3306v1 2012-08-31,A Piggyback resistive Micromegas,"A novel read-out architecture has been developed for the Micromegas detector. The anode element is made of a resistive layer on a ceramic substrate. The detector part is entirely separated from the read-out element. Without significant loss, signals are transmitted by capacitive coupling to the read-out pads. The detector provides high gas gain, good energy resolution and the resistive layer assures spark protection to the electronics. This assembly could be combined with modern pixel array electronic ASICs. This readout organization is free on how the pixels are designed, arranged and connected. We present first results taken with a MediPix read-out chip.",1208.6525v2 2012-10-18,Design and Simulation of Molecular Nonvolatile Single-Electron Resistive Switches,"We have carried out a preliminary design and simulation of a single-electron resistive switch based on a system of two linear, parallel, electrostatically-coupled molecules: one implementing a single-electron transistor and another serving as a single-electron trap. To verify our design, we have performed a theoretical analysis of this ""memristive"" device, based on a combination of ab-initio calculations of the electronic structures of the molecules and the general theory of single-electron tunneling in systems with discrete energy spectra. Our results show that such molecular assemblies, with a length below 10 nm and a footprint area of about 5 nm$^2$, may combine sub-second switching times with multi-year retention times and high ($> 10^3$) ON/OFF current ratios, at room temperature. Moreover, Monte Carlo simulations of self-assembled monolayers (SAM) based on such molecular assemblies have shown that such monolayers may also be used as resistive switches, with comparable characteristics and, in addition, be highly tolerant to defects and stray offset charges.",1210.5253v1 2012-12-11,"Anisotropic magnetization, resistivity and heat capacity of single crystalline R3Ni2-xSn7 (R = La, Ce, Pr and Nd)","We present a detailed study of R3Ni2-xSn7 (R = La, Ce, Pr and Nd) single crystals by measurements of crystal structure, stoichiometry, temperature dependent magnetic susceptibility, magnetization, electrical resistivity, magnetoresistance, and specific heat. This series forms with partial Ni occupancy with x varying from ~ 0.1 for R = La to ~0.7 for R = Nd. The electrical resistivity of this series follows metallic behavior at high temperatures. Determination of clear anisotropies as well as antiferromagnetic ordering temperatures for R3Ni2-xSn7 (R = Ce, Pr and Nd) have been made. For Pr3Ni1.56Sn7 and Nd3Ni1.34Sn7, multiple magnetic transitions take place upon cooling. Metamagnetic transitions in this family (R = Ce, Pr and Nd) were detected for applied magnetic fields below 70 kOe. An H-T phase diagram of Ce3Ni1.69Sn7 was assembled to shed light on its low field properties and to rule out possible quantum critical effects.",1212.2542v1 2013-01-21,Transparent conducting silver nanowire networks,"We present a transparent conducting electrode composed of a periodic two-dimensional network of silver nanowires. Networks of Ag nanowires are made with wire diameters of 45-110 nm and pitch of 500, 700 and 1000 nm. Anomalous optical transmission is observed, with an averaged transmission up to 91% for the best transmitting network and sheet resistances as low as 6.5 {\Omega}/sq for the best conducting network. Our most dilute networks show lower sheet resistance and higher optical transmittance than an 80 nm thick layer of ITO sputtered on glass. By comparing measurements and simulations we identify four distinct physical phenomena that govern the transmission of light through the networks: all related to the excitation of localized surface plasmons and surface plasmon polaritons on the wires. The insights given in this paper provide the key guidelines for designing high-transmittance and low-resistance nanowire electrodes for optoelectronic devices, including thin-film solar cells. For these latter, we discuss the general design principles to use the nanowire electrodes also as a light trapping scheme.",1301.4834v1 2013-01-25,The Role of the Equation of State in Resistive Relativistic Magnetohydrodynamics,"We have investigated the role of the equation of state in resistive relativistic magnetohydrodynamics using a newly developed resistive relativistic magnetohydrodynamic code. A number of numerical tests in one-dimension and multi-dimensions are carried out in order to check the robustness and accuracy of the new code. The code passes all the tests in situations involving both small and large uniform conductivities. Equations of state which closely approximate the single-component perfect relativistic gas are introduced. Results from selected numerical tests using different equations of state are compared. The main conclusion is that the choice of the equation of state as well as the value of the electric conductivity can result in considerable dynamical differences in simulations involving shocks, instabilities, and magnetic reconnection.",1301.6052v1 2013-01-28,On conditions of negativity of friction resistance for non-stationary modes of blood flow and possible mechanism of affecting of environmental factors on energy effectiveness of cardio-vascular system functioning,"It is shown that initiated by action of molecular viscosity impulse flow, directed usually from the moving fluid to limiting it solid surface, can, under certain conditions, turn to zero and get negative values in the case of non-stationary flow caused by alternating in time longitudinal (along the pipe axis) pressure gradient. It is noted that this non-equilibrium mechanism of negative friction resistance in the similar case of pulsating blood flow in the blood vessels, in addition to the stable to turbulent disturbances swirled blood flow structure providing, can also constitute hydro-mechanical basis of the observed but not explained yet paradoxically high energy effectiveness of the normal functioning of the cardio-vascular system (CVS). We consider respective mechanism of affecting on the stability of the normal work of CVS by environmental variable factors using shifting of hydro-dynamic mode with negative resistance realization range boundaries and variation of linear hydro-dynamic instability leading to the structurally stable swirled blood flow organization.",1301.6603v1 2013-02-18,Resistive wall mode and neoclassical tearing mode coupling in rotating tokamak plasmas,"A model system of equations has been derived to describe a toroidally rotating tokamak plasma, unstable to Resistive Wall Modes (RWMs) and metastable to Neoclassical Tearing Modes (NTMs), using a linear RWM model and a nonlinear NTM model. If no wall is present, the NTM growth shows the typical threshold/saturation island widths, whereas a linearly unstable kink mode grows exponentially in this model plasma system. When a resistive wall is present, the growth of the linearly unstable RWM is accelerated by an unstable island: a form of coupled RWM-NTM mode. Crucially, this coupled system has no threshold island width, giving the impression of a triggerless NTM, observed in high beta tokamak discharges. Increasing plasma rotation at the island location can mitigate its growth, decoupling the modes to yield a conventional RWM with no threshold width.",1302.4250v2 2013-03-21,On-sample water content measurement for a complete local monitoring in triaxial testing of unsaturated soils,"To provide a complete local monitoring of the state of an unsaturated soil sample during triaxial testing, a local water content measurement device was adapted to a triaxial device comprising the measurement of local displacements (Hall effect transducers) and suction (High capacity transducer). Water content was locally monitored by means of a resistivity probe. The water content/resistivity calibration curves of an intact natural unsaturated loess from Northern France extracted by block sampling at two depths (1 and 3.3 m) were carefully determined, showing good accuracy and repeatability. The validity of two models giving the resistivity of unsaturated soils with respect to their water content was examined.",1303.5348v1 2013-07-02,Structure of Intratumor Heterogeneity: Is Cancer Hedging Its Bets?,"Development of resistance limits transferability of most anticancer therapies into curative treatment and understanding mechanisms beyond it remains a big challenge. Many high resolution experimental observations show enormous intratumor heterogeneity at molecular, genetic and cellular levels which is made responsible for emerging resistance to therapy. Therefore, researchers search techniques to influence development of intratumor heterogeneity, which requires understanding its role within the context of integrative, logically consistent, framework, such as evolutionary theory. Although it is agreed that intratumor heterogeneity increases probability of the emergence of therapy resistant clones, more instructive role of its structure in the process of cancer dynamics and metastasis is needed. In the paper, intratumor heterogeneity is viewed as a product of two, in general stochastic, processes, evolutionary optimization and changing environment, respectively. In evolutionary theory, common risk-diversifying strategy displayed by isogenic populations in unpredictably changing environments is bet-hedging. We suggest, that the structure of intratumor heterogeneity is evolutionary trait evolving to maximize the clonal fitness in changing (or uncertain) environment and that its structure corresponds to bet-hedging strategy. We advocate our view by reviewing and combining important cancer relevant concepts.",1307.0607v1 2013-07-25,Memory Effect and Triplet Pairing Generation in the Superconducting Exchange Biased Co/CoOx/Cu41Ni59/Nb/Cu41Ni59 Layered Heterostructure,"We fabricated a nanolayered hybrid superconductor-ferromagnet spin-valve structure, the resistive state of which depends on the preceding magnetic field polarity. The effect is based on a strong exchange bias (about -2 kOe) on a diluted ferromagnetic copper-nickel alloy and generation of a long range odd in frequency triplet pairing component. The difference of high and low resistance states at zero magnetic field is 90% of the normal state resistance for a transport current of 250 {\mu}A and still around 42% for 10 {\mu}A. Both logic states of the structure do not require biasing fields or currents in the idle mode.",1307.6742v1 2013-08-28,Tunneling at $ν_T=1$ in Quantum Hall Bilayers,"Interlayer tunneling measurements in the strongly correlated bilayer quantized Hall phase at $\nu_T=1$ are reported. The maximum, or critical current for tunneling at $\nu_T=1$, is shown to be a well-defined global property of the coherent phase, insensitive to extrinsic circuit effects and the precise configuration used to measure it, but also exhibiting a surprising scaling behavior with temperature. Comparisons between the experimentally observed tunneling characteristics and a recent theory are favorable at high temperatures, but not at low temperatures where the tunneling closely resembles the dc Josephson effect. The zero-bias tunneling resistance becomes extremely small at low temperatures, vastly less than that observed at zero magnetic field, but nonetheless remains finite. The temperature dependence of this tunneling resistance is similar to that of the ordinary in-plane resistivity of the quantum Hall phase.",1308.6269v2 2013-10-22,The Effect of Toroidal Magnetic Field on Thickness of a Viscose-Resistive Hot Accreting Flow,"By taking into account the effect of toroidal magnetic field and its correspond heating, we determine the thickness of advection-dominated accretion flows. We consider an axisymetric, rotating, steady viscous-resistive, magnetized accretion flow under an advection dominated stage. The dominant mechanism of energy dissipation is assumed to be turbulence viscosity and magnetic diffusivity. We adopt a self-similar assumption in the radial direction to obtain the dynamical quantities, that is, radial, azimuthal, sound and Alfv\' en velocities. Our results show the vertical component of magnetic force acts in the opposite direction of gravity and compresses the disc, thus compared with the non-magnetic case, in general the disc half-thikness, $\Delta\theta$, significantly is reduced. On the other hand, two parameters, appearing due to action of magnetic field and reaction of the flow, affect the disc thickness. The first one, $\beta_0$, showing the magnetic field strength at the equatorial plane, decreases $\Delta\theta$. The other one, $\eta_0$ is the magnetic resistivity parameter and when it increases, $\Delta\theta$ increases, too.",1310.6317v1 2014-02-13,Theory of measurements of d.c. and a.c. resistivity in anisotropic superconductors in tilted magnetic fields,"The vortex dynamics of uniaxial anisotropic superconductors with arbitrary angles between the magnetic field, the applied current and the anisotropy axis is theoretically studied, by focusing on the models for electrical transport experiments in the linear regime. The vortex parameters, such as the viscous drag, the vortex mobility and the pinning constant (in the weak point pinning regime), together with the vortex motion resistivity, are derived in tensor form by considering the very different free flux flow and pinned Campbell regimes. The results are extended to high frequency regimes where additional effects like thermal depinning/creep take place. The applicability to the various tensor quantities of the well-known scaling laws for the angular dependence on the field orientation is commented, illustrating when and with which cautions the scaling approach can be used to discriminate between intrinsic and extrinsic effects. It is shown that the experiments do not generally yield the intrinsic values of the vortex parameters and vortex resistivities. Explicit expressions relating measured and intrinsic quantities are given and their use exemplified in data analyses of angular measurements.",1402.3164v1 2014-05-05,Colossal negative magnetoresistance in a 2D electron gas,"We report on a colossal negative magnetoresistance (MR) in GaAs/AlGaAs quantum well which, at low temperatures, is manifested by a drop of the resistivity by more than an order of magnitude at a magnetic field $B \approx 1$ kG. In contrast to MR effects discussed earlier, the MR reported here is not parabolic, even at small $B$, and persists to much higher in-plane magnetic fields and temperatures. Remarkably, the temperature dependence of the resistivity at $B \approx 1$ kG is linear over the entire temperature range studied (from 1 to 30 K) and appears to coincide with the high-temperature limit of the zero-field resistivity, hinting on the important role of acoustic phonons.",1405.1090v1 2014-09-30,Formation of magnetic moments and resistance upturn at grain boundaries of two-dimensional electron systems,"Electronic correlations control the normal state of bulk high-Tc cuprates. Strong correlations also suppress the charge transport through cuprate grain boundaries (GBs). The question then arises if these correlations can produce magnetic states at cuprate GBs. We analyze the formation of local magnetic moments at the GB of a correlated two-dimensional electron systems which is represented by an inhomogeneous Hubbard model. The model Hamiltonian is diagonalized after the implementation of a mean-field decoupling. The formation of local magnetic moments is supported by a sufficiently strong variance in the bond kinetic energies at the GB. Local scattering potentials can assist or suppress the formation of a magnetic GB state, depending on the details of their spacial distribution. Grain boundary induced stripes are formed in the vicinity the GB and decay into the bulk. Moreover, we observe the build-up of conducting channels which are confined by magnetic clusters. The grain boundary resistance increases at decreasing temperatures. This low-temperature behavior is caused by the suppression of current correlations in the state with local magnetic GB moments. The resistance upturn at low temperatures is in qualitative agreement with experiments.",1409.8559v1 2014-10-30,Magnetoresistance of layered conductors under conditions of topological phase transition,"The resistance of layered conductors with a multisheet Fermi surface (FS), in a high magnetic field, in the immediate vicinity of Lifshic's topological transition when the separate FS sheets are drown together by an external action, pressure in part (and eventual change of the FS connectivity) is studied theoretically. Analysis of magnetoresistance near topological transition is illustrated for the case of FS in the shape of lightly corrugated cylinder and two corrugated planes distributed with a repeated period in the pulse space. It yields, that as the FS plane sheets approach sufficiently the cylinder, the charge carriers produce a magnetic breakdown of one FS sheet to another, decreasing a sharp anisotropy of magnetoresistance to the in-plane current. Instead of square increase with a magnetic field, the slower resistance growth remains linear in the field within a broad magnetic-field range. In the intimate vicinity of topological transition, when the energy gap between FS layers is negligibly small, the resistance is saturated.",1410.8330v1 2014-11-10,The Resistive-WELL detector: a compact spark-protected single amplification-stage MPGD,"In this work we present a novel idea for a compact spark-protected single amplification stage Micro-Pattern Gas Detector (MPGD). The detector amplification stage, realized with a structure very similar to a GEM foil, is embedded through a resistive layer in the readout board. A cathode electrode, defining the gas conversion/drift gap, completes the detector mechanics. The new structure, that we call Resistive-WELL (R-WELL), has some characteristics in common with previous MPGDs, such as C.A.T. and WELL, developed more than ten years ago. The prototype object of the present study has been realized in the 2009 by TE-MPE-EM Workshop at CERN. The new architecture is a very compact MPGD, robust against discharges and exhibiting a large gain ($\sim$6$\times$10$^3$), simple to construct and easy for engineering and then suitable for large area tracking devices as well as huge calorimetric apparata.",1411.2466v1 2015-01-01,Fast Generation of Random Spanning Trees and the Effective Resistance Metric,"We present a new algorithm for generating a uniformly random spanning tree in an undirected graph. Our algorithm samples such a tree in expected $\tilde{O}(m^{4/3})$ time. This improves over the best previously known bound of $\min(\tilde{O}(m\sqrt{n}),O(n^{\omega}))$ -- that follows from the work of Kelner and M\k{a}dry [FOCS'09] and of Colbourn et al. [J. Algorithms'96] -- whenever the input graph is sufficiently sparse. At a high level, our result stems from carefully exploiting the interplay of random spanning trees, random walks, and the notion of effective resistance, as well as from devising a way to algorithmically relate these concepts to the combinatorial structure of the graph. This involves, in particular, establishing a new connection between the effective resistance metric and the cut structure of the underlying graph.",1501.00267v1 2015-03-16,On Resistive Networks of Constant Power Devices,"This brief examines the behavior of DC circuits comprised of resistively interconnected constant power devices, as may arise in DC microgrids containing micro-sources and constant power loads. We derive a sufficient condition for all operating points of the circuit to lie in a desirable set, where the average nodal voltage level is high and nodal voltages are tightly clustered near one another. Our condition has the elegant physical interpretation that the ratio of resistive losses to total injected power should be small compared to a measure of network heterogeneity, as quantified by a ratio of conductance matrix eigenvalues. Perhaps surprisingly, the interplay between the circuit topology, branch conductances and the constant power devices implicitly defines a nominal voltage level for the circuit, despite the explicit absence of voltage-regulated nodes.",1503.04769v1 2015-08-04,"Electron Viscosity, Current Vortices and Negative Nonlocal Resistance in Graphene","Quantum-critical states of diverse strongly correlated systems are predicted to feature universal collision-dominated transport resembling that of viscous fluids. However, investigation of these phenomena has been hampered by the lack of known macroscopic signatures of the hydrodynamic regime at criticality. Here we identify vorticity as such a signature and link it with an easily verifiable striking macroscopic transport behavior. Produced by the viscous flow, vorticity can drive electric current against an applied field, resulting in a negative nonlocal voltage. We argue that the latter may play the same role for the viscous regime as zero electrical resistance does for superconductivity. Besides offering a diagnostic of viscous transport which distinguishes it from ohmic currents, the sign-changing electrical response affords a robust tool for directly measuring the viscosity-to-resistivity ratio. The strongly interacting electron-hole plasma in high-mobility graphene provides a bridge between quantum-criticality and the wealth of fluid mechanics phenomena.",1508.00836v2 2015-10-13,Charge order and suppression of superconductivity in HgBa2CuO4 at high pressures,"New insight into the superconducting properties of HgBa2CuO4 (Hg-1201) cuprates is provided by combined measurements of the electrical resistivity and single crystal X-ray diffraction under pressure. The changes induced by increasing pressure up to 20GPa in optimally doped single crystals were investigated. The resistivity measurements as a function of temperature show a metallic behavior up to ~10GPa that gradually passes to an insulating state, typical of charge ordering, that totally suppresses superconductivity above 13GPa. The changes in resistivity are accompanied by the apparition of sharp Bragg peaks in the X-ray diffraction patterns indicating that the charge ordering is accompanied by a 3D oxygen ordering appearing at 10GPa of wavevector [0.25, 0, L]. As pressure induces a charge transfer of about 0.02 at 10GPa, our results are the first observation of charge order competing with superconductivity that develops in the over-doped region of the phase diagram of a cuprate.",1510.03750v1 2015-11-15,Synchronization of two memristive coupled van der Pol oscillators,"The objective of this paper is to explore the possibility to couple two van der Pol (vdP) oscillators via a resistance-capacitance (RC) network comprising a Ag-TiOx-Al memristive device. The coupling was mediated by connecting the gate terminals of two programmable unijunction transistors (PUTs) through the network. In the high resistance state (HRS) the memresistance was in the order of MOhm leading to two independent selfsustained oscillators characterized by the different frequencies f1 and f2 and no phase relation between the oscillations. After a few cycles and in dependency of the mediated pulse amplitude the memristive device switched to the low resistance state (LRS) and a frequency adaptation and phase locking was observed. The experimental results are underlined by theoretically considering a system of two coupled vdP equations. The presented neuromorphic circuitry conveys two essentials principle of interacting neuronal ensembles: synchronization and memory. The experiment may path the way to larger neuromorphic networks in which the coupling parameters can vary in time and strength and are realized by memristive devices.",1511.06363v1 2015-12-07,Universality of DC Electrical Conductivity from Holography,"We propose a universal formula of dc electrical conductivity in rotational- and translational- symmetries breaking systems via the holographic duality. This formula states that the ratio of the determinant of the dc electrical conductivities along any spatial directions to the black hole area density in zero-charge limit has a universal value. As explicit illustrations, we give several examples elucidating the validation of this formula: We construct an anisotropic black brane solution, which yields linear in temperature for the in-plane resistivity and insulating behavior for the out-of-plane resistivity; We also construct a spatially isotropic black brane solution that both the linear-T and quadratic-T contributions to the resistivity can be realized.",1512.01917v3 2016-01-26,Observation of An Anisotropic Wigner Crystal,"We report a new correlated phase of two-dimensional charged carriers in high magnetic fields, manifested by an anisotropic insulating behavior at low temperatures. It appears near Landau level filling factor $\nu=1/2$ in hole systems confined to wide GaAs quantum wells when the sample is tilted in magnetic field to an intermediate angle. The parallel field component ($B_{||}$) leads to a crossing of the lowest two Landau levels, and an elongated hole wavefunction in the direction of $B_{||}$. Under these conditions, the in-plane resistance exhibits an insulating behavior, with the resistance along $B_{||}$ more than 10 times smaller than the resistance perpendicular to $B_{||}$. We interpret this anisotropic insulating phase as a two-component, striped Wigner crystal.",1601.07135v1 2016-02-05,Investigating Reliability Aspects of Memristor based RRAM with Reference to Write Voltage and Frequency,"In this paper, we report the effect of write voltage and frequency on memristor based Resistive Random Access Memory (RRAM). The above said parameters have been investigated on the linear drift model of memristor. With a variation of write voltage from 0.2V to 1.2V and a subsequent frequency modulation from 1, 2, 4, 10, 100 and 200 Hz the corresponding effects on memory window, Low Resistance State (LRS) and High Resistance State (HRS) have been reported. Thus the lifetime ({\tau}) reliability analysis of memristor based RRAM is carried out using above results. It is found that, the HRS is independent of write voltage, whereas LRS shows dependency on write voltage and frequency. The simulation results showcase that the memristor possess higher memory window and lifetime ({\tau}) in the higher voltage with lower frequency region, which has been attributed to the fewer data losses in the memory architecture.",1602.01947v1 2016-06-23,Device and Circuit Interaction Analysis of Stochastic Behaviors in Cross-Point RRAM Arrays,"Stochastic behaviors of resistive random access memory (RRAM) play an important role in the design of cross-point memory arrays. A Monte Carlo compact model of oxide RRAM is developed and calibrated with experiments on various device stack configurations. With Monte Carlo SPICE simulations, we show that an increase in array size and interconnect wire resistance will statistically deteriorate write functionality. Write failure probability (WFP) has an exponential dependency on device uniformity and supply voltage (VDD), and the array bias scheme is a key knob. Lowering array VDD leads to higher effective energy consumption (EEC) due to the increase in WFP when the variation statistics are included in the analysis. Random-access simulations indicate that data sparsity statistically benefits write functionality and energy consumption. Finally, we show that a pseudo-sub-array topology with uniformly distributed pre-forming cells in the pristine high resistance state is able to reduce both WFP and EEC, enabling higher net capacity for memory circuits due to improved variation tolerance.",1606.07457v3 2016-07-05,The Importance of the Electron Mean Free Path for Superconducting RF Cavities,"Impurity-doping is an exciting new technology in the field of SRF, producing cavities with record-high quality factor $Q_0$ and BCS surface resistance that decreases with increasing RF field. Recent theoretical work has offered a promising explanation for this anti-Q-slope, but the link between the decreasing surface resistance and the short mean free path of doped cavities has remained elusive. In this work we investigate this link, finding that the magnitude of this decrease varies directly with the mean free path: shorter mean free paths correspond with stronger anti-Q-slopes. We draw a theoretical connection between the mean free path and the overheating of the quasiparticles, which leads to the reduction of the anti-Q-slope towards the normal Q-slope of long-mean-free-path cavities. We also investigate the sensitivity of the residual resistance to trapped magnetic flux, a property which is greatly enhanced for doped cavities, and calculate an optimal doping regime for a given amount of trapped flux.",1607.01411v2 2016-08-01,"Graphene-based, mid-infrared, room-temperature pyroelectric bolometers with ultrahigh temperature coefficient of resistance","Graphene is ideally suited for photonic and optoelectronic applications, with a variety of photodetectors (PDs) in the visible, near-infrared (NIR), and THz reported to date, as well as thermal detectors in the mid-infrared (MIR). Here, we present a room temperature-MIR-PD where the pyroelectric response of a LiNbO3 crystal is transduced with high gain (up to 200) into resistivity modulation for graphene, leading to a temperature coefficient of resistance up to 900%/K, two orders of magnitude higher than the state of the art, for a device area of 300x300um2. This is achieved by fabricating a floating metallic structure that concentrates the charge generated by the pyroelectric substrate on the top-gate capacitor of the graphene channel. This allows us to resolve temperature variations down to 15umK at 1 Hz, paving the way for a new generation of detectors for MIR imaging and spectroscopy",1608.00569v1 2016-08-07,Anisotropic physical properties and pressure dependent magnetic ordering of CrAuTe$_4$,"Systematic measurements of temperature dependent magnetization, resistivity and angle-resolved photoemission spectroscopy (ARPES) at ambient pressure as well as resistivity under pressures up to 5.25 GPa were conducted on single crystals of CrAuTe$_4$. Magnetization data suggest that magnetic moments are aligned antiferromagnetically along the crystallographic $c$-axis below $T_\textrm{N}$ = 255 K. ARPES measurements show band reconstruction due to the magnetic ordering. Magnetoresistance data show clear anisotropy, and, at high fields, quantum oscillations. The Neel temperature decreases monotonically under pressure, decreasing to $T_\textrm{N}$ = 236 K at 5.22 GPa. The pressure dependencies of (i) $T_\textrm{N}$, (ii) the residual resistivity ratio, and (iii) the size and power-law behavior of the low temperature magnetoresistance all show anomalies near 2 GPa suggesting that there may be a phase transition (structural, magnetic, and/or electronic) induced by pressure. For pressures higher than 2 GPa a significantly different quantum oscillation frequency emerges, consistent with a pressure induced change in the electronic states.",1608.02213v2 2016-08-11,Anisotropic and strong negative magneto-resistance in the three-dimensional topological insulator Bi2Se3,"We report on high-field angle-dependent magneto-transport measurements on epitaxial thin films of Bi2Se3, a three-dimensional topological insulator. At low temperature, we observe quantum oscillations that demonstrate the simultaneous presence of bulk and surface carriers. The magneto- resistance of Bi2Se3 is found to be highly anisotropic. In the presence of a parallel electric and magnetic field, we observe a strong negative longitudinal magneto-resistance that has been consid- ered as a smoking-gun for the presence of chiral fermions in a certain class of semi-metals due to the so-called axial anomaly. Its observation in a three-dimensional topological insulator implies that the axial anomaly may be in fact a far more generic phenomenon than originally thought.",1608.03615v1 2016-08-15,Effect of electrical properties of glass electrodes on the performance of RPC detectors for the INO-ICAL experiment,"The India-based Neutrino Observatory (INO) collaboration has chosen glass Resistive Plate Chambers (RPCs) as the active detector elements for the Iron Calorimeter (ICAL) experiment. In the present work, we study the electrical properties such as bulk resistivity and relative permittivity of the glasses from two different manufacturers and compared the performances of RPCs built using these glasses. We conclude that the glass electrodes with larger bulk resistivy and permittivity are better suited for manufacturing RPCs for the ICAL experiment, as these detectors could be operated at lower bias currents and voltages, and produce better time resolutions compared to those built with glass electrodes of smaller bulk resistivity and permittivity.",1608.04230v1 2016-12-02,Random walk hitting times and effective resistance in sparsely connected Erdős-Rényi random graphs,"We prove expectation and concentration results for the following random variables on an Erd\H{o}s-R\'enyi random graph $\mathcal{G}\left(n,p\right)$ in the sparsely connected regime $\log n + \log\log \log n \leq np < n^{1/10}$: effective resistances, random walk hitting and commute times, the Kirchoff index, cover cost, random target times, the mean hitting time and Kemeny's constant. For the effective resistance between two vertices our concentration result extends further to $np\geq c\log n, \; c>0$. To achieve these results, we show that a strong connectedness property holds with high probability for $\mathcal{G}(n,p)$ in this regime.",1612.00731v2 2016-12-26,Analysis of claims that the brain extracellular impedance is high and non-resistive,"Numerous measurements in the brain of the impedance between two extracellular electrodes have shown that it is approximately resistive in the range of biological interest, $<10\,$kHz, and has a value close to that expected from the conductivity of physiological saline and the extracellular volume fraction in brain tissue. Recent work from the group of Claude B\'edard and Alain Destexhe has claimed that the impedance of the extracellular space is some three orders of magnitude greater than these values and also displays a $1/\sqrt{f}$ frequency dependence (above a low-frequency corner frequency). Their measurements were performed between an intracellular electrode and an extracellular electrode. It is argued that they incorrectly extracted the extracellular impedance because of an inaccurate representation of the large, confounding impedance of the neuronal membrane. In conclusion, no compelling evidence has been provided to undermine the well established and physically plausible consensus that the brain extracellular impedance is low and approximately resistive",1612.08457v5 2017-02-02,Influence of thermal boundary conditions on the current-driven resistive transition in $\mathbf{VO_2}$ microbridges,"We investigate the resistive switching behaviour of $\mathrm{VO_2}$ microbridges under current bias as a function of temperature and thermal coupling with the heat bath. Upon increasing the electrical current bias, the formation of the metallic phase can progress smoothly or through sharp jumps. The magnitude and threshold current values of these sharp resistance drops show random behaviour and are dramatically influenced by thermal dissipation conditions. Our results also evidence how the propagation of the metallic phase induced by electrical current in $\mathrm{VO_2}$, and thus the shape of the resulting high-conductivity path, are not predictable. We discuss the origin of the switching events through a simple electro-thermal model based on the domain structure of $\mathrm{VO_2}$ films that can be useful to improve the stability and controllability of future $\mathrm{VO_2}$-based devices.",1702.00805v1 2017-06-05,Enhancement of superconductivity in NbN nanowires by negative electron-beam lithography with positive resist,"We performed comparative experimental investigation of superconducting NbN nanowires which were prepared by means of positive-and negative electron-beam lithography with the same positive tone Poly-methyl-methacrylate (PMMA) resist. We show that nanowires with a thickness 4.9 nm and widths less than 100 nm demonstrate at 4.2 K higher critical temperature and higher density of critical and retrapping currents when they are prepared by negative lithography. Also the ratio of the experimental critical-current to the depairing critical current is larger for nanowires prepared by negative lithography. We associate the observed enhancement of superconducting properties with the difference in the degree of damage that nanowire edges sustain in the lithographic process. A whole range of advantages which is offered by the negative lithography with positive PMMA resist ensures high potential of this technology for improving performance metrics of superconducting nanowire singe-photon detectors.",1706.01289v2 2017-09-26,Timing and Charge measurement of single gap Resistive Plate Chamber Detectors for INO-ICAL Experiment,"The recently approved India-based Neutrino Observatory will use the world's largest magnet to study atmospheric muon neutrinos. The 50 kiloton Iron Calorimeter consists of iron alternating with single-gap resistive plate chambers. A uniform magnetic field of $\sim$1.5 T is produced in the iron using toroidal-shaped copper coils. Muon neutrinos interact with the iron target to produce charged muons, which are detected by the resistive plate chambers, and tracked using orthogonal pick up strips. Timing information for each layer is used to discriminate between upward and downward traveling muons. The design of the readout electronics for the detector depends critically on an accurate model of the charge induced by the muons, and the dependence on bias voltages. In this paper, we present timing and charge response measurements using prototype detectors under different operating conditions. We also report the effect of varying gas mixture, particularly $SF_6$, on the timing response.",1709.08946v1 2017-10-30,Analysis of the measurements of anisotropic a.c. vortex resistivity in tilted magnetic fields,"Measurements of the high-frequency complex resistivity in superconductors are a tool often used to obtain the vortex parameters, such as the vortex viscosity, the pinning constant and the depinning frequency. In anisotropic superconductors, the extraction of these quantities from the measurements faces new difficulties due to the tensor nature of the electromagnetic problem. The problem is specifically intricate when the magnetic field is tilted with respect to the crystallographic axes. Partial solutions exist in the free-flux-flow (no pinning) and Campbell (pinning dominated) regimes. In this paper we develop a full tensor model for the vortex motion complex resistivity, including flux-flow, pinning, and creep. We give explicit expressions for the tensors involved. We obtain that, despite the complexity of the physics, some parameters remain scalar in nature. We show that under specific circumstances the directly measured quantities do not reflect the true vortex parameters, and we give procedures to derive the true vortex parameters from measurements taken with arbitrary field orientations. Finally, we discuss the applicability of the angular scaling properties to the measured and transformed vortex parameters and we exploit these properties as a tool to unveil the existence of directional pinning.",1710.11485v1 2018-03-06,Effect of charge ordering on the electrical properties and magnetoresistance of manganites,"The Monte Carlo Ferromagnetic Ising model was used to study the electrical properties of manganese oxides due to the charge ordering phase occurring at doping, x = 0.5. The half-doped manganites have an insulator antiferromagnetic ground state. We calculated the internal energy, specific heat, resistivity and the magneto-resistance, MR, with parallel and anti-parallel applied magnetic fields. Our simulation reveals that the resistivity decreases exponentially and the electric current increases with increasing temperature according the free charge increase, to transport from an insulator to conductor phase. The magnetoresistance has negative small values with parallel magnetic field but has positive high values with unti-parallel magnetic field. The obtained semiconductor-metal transition behavior candidates the half-doped manganites to be very good semiconductors diode junctions.",1803.02283v1 2018-05-21,Holographic DC Conductivity for Backreacted Nonlinear Electrodynamics with Momentum Dissipation,"We consider a holographic model with the charge current dual to a general nonlinear electrodynamics (NLED) field. Taking into account the backreaction of the NLED field on the geometry and introducing axionic scalars to generate momentum dissipation, we obtain expressions for DC conductivities with a finite magnetic field. The properties of the in-plane resistance are examined in several NLED models. For Maxwell-Chern-Simons electrodynamics, negative magneto-resistance and Mott-like behavior could appear in some parameter space region. Depending on the sign of the parameters, we expect the NLED models to mimic some type of weak or strong interactions between electrons. In the latter case, negative magneto-resistance and Mott-like behavior can be realized at low temperatures. Moreover, the Mott insulator to metal transition induced by a magnetic field is also observed at low temperatures.",1805.07913v2 2018-06-23,Magnetic and magnetoresistive behavior of the ferromagnetic heavy fermion YbNi$_2$,"We present a study on the magnetic susceptibility $\chi(T)$ and electrical resistance, as a function of temperature and magnetic field $R(T,H)$, of the ferromagnetic heavy fermion YbNi$_2$. The X-ray diffraction analysis shows that the synthesized polycrystalline samples crystallizes in the cubic Laves phase structure C15, with a spatial group $Fd\overline{3}m$. The magnetic measurements indicate a ferromagnetic behavior with transition temperature at 9 K. The electrical resistance is metallic-like at high temperatures and no signature of Kondo effect was observed. In the ferromagnetic state, the electrical resistance can be justified by electron-magnon scattering considering the existence of an energy gap in the magnonic spectrum. The energy gap was determined for various applied magnetic fields. Magnetoresistance as a function of applied magnetic field, subtracted from the $R(T,H)$ curves at several temperatures, is negative from 2 K until about 40 K for all applied magnetic fields. The negative magnetoresistance originates from the suppression of magnetic disorder by the magnetic field.",1806.08881v1 2018-09-17,Resisting Selfish Mining Attacks in the Bicomp,"Selfish mining, which is an attack on the integrity of the Bitcoin network, was first proposed by Cornell researchers Emin Gun Sirer and Ittay Eyal in 2013. Selfish mining attack also exists in most Nakamoto consensus protocols. Generally speaking, selfish mining strategy can comprise a Nakamoto consensus system with less than 25% mining power of the whole system. We have discussed how the Bicomp can resist selfish mining in our former paper ""Bicomp: A Bilayer Scalable Nakamoto Consensus Protocol"". In this technical report, we give a detailed derivation on the conditions a selfish attacker should meet to earn more revenues through selfish mining. And we also get a conclusion that through adjusting macroblock difficulties together with tenure lengths, the Bicomp protocol has high resistant towards selfish mining.",1809.06289v1 2017-03-30,Deep Neural Network Optimized to Resistive Memory with Nonlinear Current-Voltage Characteristics,"Artificial Neural Network computation relies on intensive vector-matrix multiplications. Recently, the emerging nonvolatile memory (NVM) crossbar array showed a feasibility of implementing such operations with high energy efficiency, thus there are many works on efficiently utilizing emerging NVM crossbar array as analog vector-matrix multiplier. However, its nonlinear I-V characteristics restrain critical design parameters, such as the read voltage and weight range, resulting in substantial accuracy loss. In this paper, instead of optimizing hardware parameters to a given neural network, we propose a methodology of reconstructing a neural network itself optimized to resistive memory crossbar arrays. To verify the validity of the proposed method, we simulated various neural network with MNIST and CIFAR-10 dataset using two different specific Resistive Random Access Memory (RRAM) model. Simulation results show that our proposed neural network produces significantly higher inference accuracies than conventional neural network when the synapse devices have nonlinear I-V characteristics.",1703.10642v1 2019-02-01,Achieving sub-1 Ohm-mm Non-Recess S/D Contact Resistance in GaN HEMTs Utilizing Simple CMOS Compatible La/Ti/Al/Ti Metal Contacts,"In this paper, we report the use of lanthanum (La) in S/D contacts of GaN HEMTs, achieving 0.97 Ohm-mm contact resistance without S/D recess. The HEMTs show well-behaved electrical characteristics and satisfactory reliability. Our studies show that La, a CMOS compatible metal, is promising to lower GaN HEMT S/D contact resistance. La's low work function (3.5 eV) is beneficial for reducing the barrier between the metals and GaN. The Ohmic contact formation mechanism involved was shown to be different from conventional Ti/Al films. Spherical-shaped high-La regions formed near the surface during annealing. La diffuses into the AlGaN layer, and the overlap of La and Al peaks is significantly increased compared with that before annealing.",1902.00227v1 2019-02-05,Resistive dissipative magnetohydrodynamics from the Boltzmann-Vlasov equation,"We derive the equations of motion of relativistic, resistive, second-order dissipative magnetohydrodynamics from the Boltzmann-Vlasov equation using the method of moments. We thus extend our previous work [Phys. Rev. D 98, 076009 (2018)], where we only considered the non-resistive limit, to the case of finite electric conductivity. This requires keeping terms proportional to the electric field $E^\mu$ in the equations of motions and leads to new transport coefficients due to the coupling of the electric field to dissipative quantities. We also show that the Navier-Stokes limit of the charge-diffusion current corresponds to Ohm's law, while the coefficients of electrical conductivity and charge diffusion are related by a type of Wiedemann-Franz law.",1902.01699v1 2019-07-23,Magnetotransport properties of granular oxide-segregated CoPtCr films for applications in future magnetic memory technology,"Magnetotransport properties of granular oxide-segregated CoPtCr films were studied on both macroscopic and microscopic length scales by performing bulk and point-contact magnetoresistance measurements, respectively. Such a perpendicular magnetic medium is used in state-of-the-art hard disc drives and if combined with magnetoresistive phenomena (for read/write operations) may lead to a novel concept for magnetic recording with high areal density. While the bulk measurements on the films showed only small variations in dc resistance as a function of applied magnetic field (magnetoresistance of less than 0.02 %), the point-contact measurements revealed giant-magnetoresistance-like changes in resistance with up to 50,000 % ratios. The observed magnetorestive effect could be attributed to a tunnel magnetoresistance between CoPtCr grains with different coercivity. The tunneling picture of electronic transport in our granular medium was confirmed by the observation of tunneling-like current-voltage characteristics and bias dependence of magnetoresistance; both the point-contact resistance and magnetoresistance were found to decrease with the applied dc bias.",1907.09675v1 2020-02-01,Isotropically conducting (hidden) quantum Hall stripe phases in a two-dimensional electron gas,"Quantum Hall stripe (QHS) phases, predicted by the Hartree-Fock theory, are manifested in GaAs-based two-dimensional electron gases as giant resistance anisotropies. Here, we predict a ``hidden'' QHS phase which exhibits \emph{isotropic} resistivity whose value, determined by the density of states of QHS, is independent of the Landau index $N$ and is inversely proportional to the Drude conductivity at zero magnetic field. At high enough $N$, this phase yields to an Ando-Unemura-Coleridge-Zawadski-Sachrajda phase in which the resistivity is proportional to $1/N$ and to the ratio of quantum and transport lifetimes. Experimental observation of this border should allow one to find the quantum relaxation time.",2002.00154v6 2007-10-25,Simulation Methodology for Analysis of Substrate Noise Impact on Analog / RF Circuits Including Interconnect Resistance,"This paper reports a novel simulation methodology for analysis and prediction of substrate noise impact on analog / RF circuits taking into account the role of the parasitic resistance of the on-chip interconnect in the impact mechanism. This methodology allows investigation of the role of the separate devices (also parasitic devices) in the analog / RF circuit in the overall impact. This way is revealed which devices have to be taken care of (shielding, topology change) to protect the circuit against substrate noise. The developed methodology is used to analyze impact of substrate noise on a 3 GHz LC-tank Voltage Controlled Oscillator (VCO) designed in a high-ohmic 0.18 $\mu$m 1PM6 CMOS technology. For this VCO (in the investigated frequency range from DC to 15 MHz) impact is mainly caused by resistive coupling of noise from the substrate to the non-ideal on-chip ground interconnect, resulting in analog ground bounce and frequency modulation. Hence, the presented test-case reveals the important role of the on-chip interconnect in the phenomenon of substrate noise impact.",0710.4723v1 2014-01-27,Transport near the Ising-nematic quantum critical point of metals in two dimensions,"We consider two-dimensional metals near a Pomeranchuk instability which breaks 90$^\circ$ lattice rotation symmetry. Such metals realize strongly-coupled non-Fermi liquids with critical fluctuations of an Ising-nematic order. At low temperatures, impurity scattering provides the dominant source of momentum relaxation, and hence a non-zero electrical resistivity. We use the memory matrix method to compute the resistivity of this non-Fermi liquid to second order in the impurity potential, without assuming the existence of quasiparticles. Impurity scattering in the $d$-wave channel acts as a random ""field"" on the Ising-nematic order. We find contributions to the resistivity with a nearly linear temperature dependence, along with more singular terms; the most singular is the random-field contribution which diverges in the limit of zero temperature.",1401.7012v2 2016-03-21,Spin Hall effects in mesoscopic Pt films with high resistivity,"The energy efficiency of the spin Hall effects (SHE) can be enhanced if the electrical conductivity is decreased without sacrificing the spin Hall conductivity. The resistivity of Pt films can be increased to 150-300 {\mu}{\Omega}*cm by mesoscopic lateral confinement, thereby decreasing the conductivity. The SHE and inverse spin Hall effects (ISHE) in these mesoscopic Pt films are explored at 10 K by using the nonlocal spin injection/detection method. All relevant physical quantities are determined in-situ on the same substrate, and a quantitative approach is developed to characterize all processes effectively. Extensive measurements with various Pt thickness values reveal an upper limit for the Pt spin diffusion length: {\lambda}_pt<0.8 nm. The average product of {\lambda}_pt and the Pt spin Hall angle {\alpha}_H is substantial: {\alpha}_H*{\lambda}_pt=(0.142 +/- 0.040)nm for 4 nm thick Pt, though a gradual decrease is observed at larger Pt thickness. The results suggest enhanced spin Hall effects in resistive mesoscopic Pt films.",1603.06567v3 2017-05-07,Penetration of fast projectiles into resistant media: from macroscopic to subatomic projectiles,"The penetration of a fast projectile into a resistant medium is a complex process that is suitable for simple modeling, in which basic physical principles can be profitably employed. This study connects two different domains: the fast motion of macroscopic bodies in resistant media and the interaction of charged subatomic particles with matter at high energies, which furnish the two limit cases of the problem of penetrating projectiles of different sizes. These limit cases actually have overlapping applications; for example, in space physics and technology. The intermediate or mesoscopic domain finds application in atom cluster implantation technology. Here it is shown that the penetration of fast nano-projectiles is ruled by a slightly modified Newton's inertial quadratic force, namely, $F \sim v^{2-\beta}$, where $\beta$ vanishes as the inverse of projectile diameter. Factors essential to penetration depth are ratio of projectile to medium density and projectile shape.",1705.02337v2 2017-07-07,Resistance distance criterion for optimal slack bus selection,"We investigate the dependence of transmission losses on the choice of a slack bus in high voltage AC transmission networks. We formulate a transmission loss minimization problem in terms of slack variables representing the additional power injection that each generator provides to compensate the transmission losses. We show analytically that for transmission lines having small, homogeneous resistance over reactance ratios ${r/x\ll1}$, transmission losses are generically minimal in the case of a unique \textit{slack bus} instead of a distributed slack bus. For the unique slack bus scenario, to lowest order in ${r/x}$, transmission losses depend linearly on a resistance distance based indicator measuring the separation of the slack bus candidate from the rest of the network. We confirm these results numerically for several IEEE and Pegase testcases, and show that our predictions qualitatively hold also in the case of lines having inhomogeneous ${r/x}$ ratios, with optimal slack bus choices reducing transmission losses by ${10}\%$ typically.",1707.02845v1 2017-07-18,Umklapp scattering as the origin of $T$-linear resistivity in the normal state of high-$T_c$ cuprate superconductors,"The high-temperature normal state of the unconventional cuprate superconductors has resistivity linear in temperature $T$, which persists to values well beyond the Mott-Ioffe-Regel upper bound. At low-temperature, within the pseudogap phase, the resistivity is instead quadratic in $T$, as would be expected from Fermi liquid theory. Developing an understanding of these normal phases of the cuprates is crucial to explain the unconventional superconductivity. We present a simple explanation for this behavior, in terms of umklapp scattering of electrons. This fits within the general picture emerging from functional renormalization group calculations that spurred the Yang-Rice-Zhang ansatz: umklapp scattering is at the heart of the behavior in the normal phase.",1707.05666v4 2018-08-29,Resistivity of high pressure phosphorus phases,"Simple cubic (sc) black phosphorus (denoted BP), stable at P>10GPa, seems an ordinary metal. It has electron-phonon-driven superconductivity with Tc 5-10 K. The A17 phase, stable at atmospheric pressure, has a narrow gap, becomes semimetallic at P=1 GPa, and has a smooth transition to topological metal behavior at P ~ 5 GPa. The A7 phase, stable for 5>1$, magnetic field line chaos dominates the evolution of field-line topology in three-dimensional systems. Chaos has no direct role in the dissipation of energy. A large current density, $j_\eta\equiv vB/\eta$, is required for energy dissipation to be on a comparable time scale to the topological evolution. Nevertheless, chaos plus Alfv\'en wave damping explain why both timescales tend to be approximately an order of magnitude longer than the evolution timescale $a/v$. Magnetic helicity is injected onto tubes of field lines when boundary flows have vorticity. Chaos can spread but not destroy magnetic helicity. Resistivity has a negligible effect on helicity accumulation when $R_m>>1$. Helicity accumulates within a tube of field lines until the tube erupts and moves far from its original location.",2212.07487v3 2023-03-30,Partial condensation of mobile excitons in graphene multilayers,"At a large displacement field, in rhomboedral and Bernal-stacked graphene a normal paramagnetic state transitions to a correlated state. Recent experiments showed that such systems have several phase transitions as a function of the carrier density. The phase adjacent to a paramagnetic state has anomalously high resistance and reduced degeneracy of the Fermi sea. We show that both phenomena can be explained through a concept of partial intervalley exciton condensation: a fraction of particles condenses into excitons, and another forms an intervalley coherent Fermi liquid. The exciton part of the system do not contribute to the electrical current thus increasing the resistance. Within this paradigm, the increase in the resistance has entirely geometrical origin. We check validity of the phenomenological theory through numerical calculations. We also show that the quantum oscillation data should not be very different between the partial excitonic state and the intervalley coherent states suggested by other authors. Further, we suggest STM/AFM or Raman spectroscopy to have a conclusive evidence for the occurrence of the partial exciton condensation that we suggest in this paper.",2303.17350v1 2023-05-11,Dendritic Computation through Exploiting Resistive Memory as both Delays and Weights,"Biological neurons can detect complex spatio-temporal features in spiking patterns via their synapses spread across across their dendritic branches. This is achieved by modulating the efficacy of the individual synapses, and by exploiting the temporal delays of their response to input spikes, depending on their position on the dendrite. Inspired by this mechanism, we propose a neuromorphic hardware architecture equipped with multiscale dendrites, each of which has synapses with tunable weight and delay elements. Weights and delays are both implemented using Resistive Random Access Memory (RRAM). We exploit the variability in the high resistance state of RRAM to implement a distribution of delays in the millisecond range for enabling spatio-temporal detection of sensory signals. We demonstrate the validity of the approach followed with a RRAM-aware simulation of a heartbeat anomaly detection task. In particular we show that, by incorporating delays directly into the network, the network's power and memory footprint can be reduced by up to 100x compared to equivalent state-of-the-art spiking recurrent networks with no delays.",2305.06941v2 2023-07-26,$N_{\rm eff}$ constraints on light mediators coupled to neutrinos: the dilution-resistant effect,"We investigate the impact of new light particles, carrying significant energy in the early universe after neutrino decoupling, on the cosmological effective relativistic neutrino species, $N_{{\rm eff}}$. If the light particles are produced from decoupled neutrinos, $N_{{\rm eff}}$ is predominantly modified through the dilution-resistant effect. This effect arises because the energy stored in the mass of new particles is less diluted than the photon and neutrino energy as the universe expands. Our study comprehensively explores this effect, deriving $N_{{\rm eff}}$ constraints on the couplings of light mediators with neutrinos, encompassing both scalar and vector mediators. We find that the dilution-resistant effect can increase $N_{{\rm eff}}$ by 0.118 and 0.242 for scalar and vector mediators, respectively. These values can be readily reached by forthcoming CMB experiments. Upon reaching these levels, future $N_{{\rm eff}}$ constraints on the couplings will be improved by many orders of magnitude.",2307.13967v2 2023-08-08,First order transition in Pb$_{10-x}$Cu$_x$(PO$_4$)$_6$O ($0.9\frac{d}{2})$ established by Fefferman et al.(Arch. Ration. Mech. Anal., \textbf{223} (2), 677-691, 2017). Furthermore, we generalize the ill-posedness results from $H^{\frac{d}{2}-1}(\mathbb{R}^d)\times H^{\frac{d}{2}}(\mathbb{R}^d)$ to Besov spaces $B^{\frac{d}{p}-1}_{p, q}(\mathbb{R}^d)\times B^{\frac{d}{p}}_{p, q}(\mathbb{R}^d)$ and $\dot B^{\frac{d}{p}-1}_{p, q}(\mathbb{R}^d)\times \dot B^{\frac{d}{p}}_{p, q}(\mathbb{R}^d)$ for $1\le p\le\infty, q>1$. Different from the ill-posedness mechanism of the incompressible Navier-Stokes equations in $\dot B^{-1}_{\infty, q}$ \cite{B,W}, we construct an initial data such that the paraproduct terms (low-high frequency interaction) of the nonlinear term make the main contribution to the norm inflation of the magnetic field.",2404.14825v1 2012-11-05,Structure and Thermodynamical Properties of Zirconium hydrides from first-principle,"Zirconium alloys are used as nuclear fuel cladding material due to their mechanical and corrosion resistant properties together with their favorable cross-section for neutron scattering. At running conditions, however, there will be an increase of hydrogen in the vicinity of the cladding surface at the water side of the fuel. The hydrogen will diffuse into the cladding material and at certain conditions, such as lower temperatures and external load, hydrides will precipitate out in the material and cause well known embrittlement, blistering and other unwanted effects. Using phase-field methods it is now possible to model precipitation build-up in metals, for example as a function of hydrogen concentration, temperature and external load, but the technique relies on input of parameters, such as the formation energy of the hydrides and matrix. To that end, we have computed, using the density functional theory (DFT) code GPAW, the latent heat of fusion as well as solved the crystal structure for three zirconium hydride polymorphs: \delta-ZrH1.6, \gamma-ZrH, and \epsilon-ZrH2.",1211.0858v1 2019-05-16,A multi-physics methodology for four-states of matter,"We propose a numerical methodology for the simultaneous numerical simulation of four states of matter; gas, liquid, elastoplastic solids and plasma. The distinct, interacting physical processes are described by a combination of compressible, inert and reactive forms of the Euler equations, multiphase equations, elastoplastic equations and resistive MHD equations. Combinations of systems of equations are usually solved by coupling finite element for solid modelling and CFD models for fluid modelling or including material effects through boundary conditions rather than full material discretisation. Our simultaneous solution methodology lies on the recasting of all the equations in the same, hyperbolic form allowing their solution on the same grid with the same finite-volume numerical schemes. We use a combination of sharp and diffuse interface methods to track or capture material interfaces, depending on the application. The communication between the distinct systems of equations (i.e., materials separated by sharp interfaces) is facilitated by means of mixed-material Riemann solvers at the boundaries of the systems, which represent physical material boundaries. To this end we derive approximate mixed Riemann solvers for each pair of the above models based on characteristic equations. To demonstrate the applicability of the new methodology we consider a case study where we investigate the possibility of ignition of a combustible gas that lies over a liquid in a metal container that is struck by a plasma-arc akin to a lightning strike. We study the effect on the ignition of the metal container material and conductivity, of the presence of a dielectric coating, of insensitive combustible gases and sealed and pre-damaged metal surfaces.",1905.06620v1 2017-01-05,Graphene and its elemental analogue: A molecular dynamics view of fracture phenomenon,"Graphene and some graphene like two dimensional materials; hexagonal boron nitride (hBN) and silicene have unique mechanical properties which severely limit the suitability of conventional theories used for common brittle and ductile materials to predict the fracture response of these materials. This study revealed the fracture response of graphene, hBN and silicene nanosheets under different tiny crack lengths by molecular dynamics (MD) simulations using LAMMPS. The useful strength of these large area two dimensional materials are determined by their fracture toughness. Our study shows a comparative analysis of mechanical properties among the elemental analogues of graphene and suggested that hBN can be a good substitute for graphene in terms of mechanical properties. We have also found that the pre-cracked sheets fail in brittle manner and their failure is governed by the strength of the atomic bonds at the crack tip. The MD prediction of fracture toughness shows significant difference with the fracture toughness determined by Griffth's theory of brittle failure which restricts the applicability of Griffith's criterion for these materials in case of nano-cracks. Moreover, the strengths measured in armchair and zigzag directions of nanosheets of these materials implied that the bonds in armchair direction has the stronger capability to resist crack propagation compared to zigzag direction.",1701.01193v2 2022-08-04,Printing on particles: combining two-photon nanolithography and capillary assembly to fabricate multi-material microstructures,"Additive manufacturing at the micro- and nanoscale has seen a recent upsurge to suit the increasing demand for more elaborate structures. However, the integration and precise placement of multiple distinct materials at small scales remain a challenge. To this end, we combine here the directed capillary assembly of colloidal particles and two-photon direct laser writing (DLW) to realize a new class of multi-material microstructures. We use DLW both to fabricate 3D micro-templates to guide the capillary assembly of soft- and hard colloids, and to link well-defined arrangements of polystyrene or silica particles produced with capillary assembly, a process we term ""printing on particles"". The printing process is based on automated particle recognition algorithms and enables the user to connect colloids into one- and two-dimensional tailored structures, including particle clusters and lattices of varying symmetry and composition, using commercial photo-resists (IP-L or IP-PDMS). Once printed and developed, the structures can be easily harvested and re-dispersed in water. The flexibility of our method allows the combination of a wide range of materials into complex structures, which we envisage will boost the realization of new systems for a broad range of fields, including microrobotics, micromanipulation and metamaterials.",2208.02635v1 2023-10-28,Making the cut: end effects and the benefits of slicing,"Cutting mechanics in soft solids have been a subject of study for several decades, an interest fuelled by the multitude of its applications, including material testing, manufacturing, and biomedical technology. Wire cutting is the simplest model system to analyze the cutting resistance of a soft material. However, even for this simple system, the complex failure mechanisms that underpin cutting are still not completely understood. Several models that connect the critical cutting force to the radius of the wire and the key mechanical properties of the cut material have been proposed. An almost ubiquitous simplifying assumption is a state of plane (and anti-plane) strain in the material. In this paper, we show that this assumption can lead to erroneous conclusions because even such a simple cutting problem is essentially three-dimensional. A planar approximation restricts the analysis to the stress distribution in the mid-plane. However, through finite element modeling, we reveal that the maximal tensile stress - and thus the likely location of cut initiation - is in fact located in the front plane. Friction reduces the magnitude of this stress, but this detrimental effect can be counteracted by large slice-to-push (shear-to-indentation) ratios. The introduction of these end effects helps reconcile a recent controversy around the role of friction in wire cutting, for it implies that slicing can indeed reduce required cutting forces, but only if the slice-push ratio and the friction coefficient are sufficiently large. Material strain-stiffening reduces the critical indentation depth required to initiate the cut further and thus needs to be considered when cutting non-linearly elastic materials.",2310.18595v1 1996-06-27,Temperature crossovers in cuprates,"We study the temperature crossovers seen in the magnetic and transport properties of cuprates using a nearly antiferromagnetic Fermi liquid model (NAFLM). For the overdoped cuprates, we find, in agreement with earlier work, mean-field $z=2$ behavior of the magnetic variables associated with the fact that the damping rate of their spin fluctuations is essentially independent of temperature, while the resistivity exhibits a crossover from Fermi liquid behavior at low temperature to linear-in-T above a certain temperature $T_0$, due to the proximity of the quasiparticle Fermi surface to the magnetic Brillouin zone boundary. For the underdoped cuprates we argue that the sequence of crossovers identified by Barzykin and Pines in the low frequency magnetic behavior (from mean field $z=2$ at high temperatures, $T>T_{cr}$, to non-universal $z=1$ scaling behavior at intermediate $T$, $T_* 200 K scattering from fluctuating local moments describes the MR. At low fields, where the magnetisation is no longer technically saturated, we find a scaling of magnetoresistance with the square of the magnetisation, indicating that the MR due to the unwinding of spins in the conical phase arises from a similar mechanism to that in magnetic domain walls. This MR is only visible up to a temperature of about 200 K. No features can be found in the temperature or field dependence of the longitudinal resistivity that belie the presence of the underlying magnetic phase transition at TN: the marked changes in behavior are at much lower temperatures. The anomalous Hall effect has a dramatic temperature dependence in which the anomalous Hall resistivity scales quadratically with the longitudinal resistivity: comparison with anomalous Hall scaling theory shows that our system is in the intrinsic 'moderately dirty' regime. Lastly, we find evidence of a topological Hall effect of size 100 ~Ohm cm.",1402.1276v2 2014-05-16,Extracting superconducting parameters from surface resistivity by using inside temperatures of SRF cavities,"The surface resistance of an RF superconductor depends on the surface temperature, the residual resistance and various superconductor parameters, e.g. the energy gap, and the electron mean free path. These parameters can be determined by measuring the quality factor Q0 of a SRF cavity in helium-baths of different temperatures. The surface resistance can be computed from Q0 for any cavity geometry, but it is not trivial to determine the temperature of the surface when only the temperature of the helium bath is known. Traditionally, it was approximated that the surface temperature on the inner surface of the cavity was the same as the temperature of the helium bath. This is a good approximation at small RF-fields on the surface, but to determine the field dependence of Rs, one cannot be restricted to small field losses. Here we show the following: (1) How computer simulations can be used to determine the inside temperature Tin so that Rs(Tin) can then be used to extract the superconducting parameters. The computer code combines the well-known programs, the HEAT code and the SRIMP code. (2) How large an error is created when assuming the surface temperature is same as the temperature of the helium bath? It turns out that this error is at least 10% at high RF-fields in typical cases.",1405.4226v1 2014-05-23,Evolution of Anisotropic In-plane Resistivity with doping level in Ca$_{1-x}$Na$_x$Fe$_2$As$_2$ Single Crystals,"We measured the in-plane resistivity anisotropy in the underdoped Ca$_{1-x}$Na$_x$Fe$_2$As$_2$ single crystals. The anisotropy (indicated by $\rho_{\rm b} - \rho_{\rm a}$) appears below a temperature well above magnetic transition temperature $T_{\rm N}$, being positive ($\rho_{\rm b} - \rho_{\rm a} > 0$) as $x\leq$ 0.14. With increasing the doping level to $x$ = 0.19, an intersection between $\rho_{\rm b}$ and $\rho_{\rm a}$ is observed upon cooling, with $\rho_{\rm b} - \rho_{\rm a} < 0$ at low-temperature deep inside a magnetically ordered state, while $\rho_{\rm b} - \rho_{\rm a}> 0$ at high temperature. Subsequently, further increase of hole concentration leads to a negative anisotropy $\rho_{\rm b} - \rho_{\rm a} < 0$ in the whole temperature range. These results manifest that the anisotropic behavior of resistivity in the magnetically ordered state depends strongly on the competition of the contributions from different mechanisms, and the competition between the two contributions results in a complicated evolution of the anisotropy of in-plane resistivity with doping level.",1405.6199v1 2014-10-08,A Complementary Resistive Switch-based Crossbar Array Adder,"Redox-based resistive switching devices (ReRAM) are an emerging class of non-volatile storage elements suited for nanoscale memory applications. In terms of logic operations, ReRAM devices were suggested to be used as programmable interconnects, large-scale look-up tables or for sequential logic operations. However, without additional selector devices these approaches are not suited for use in large scale nanocrossbar memory arrays, which is the preferred architecture for ReRAM devices due to the minimum area consumption. To overcome this issue for the sequential logic approach, we recently introduced a novel concept, which is suited for passive crossbar arrays using complementary resistive switches (CRSs). CRS cells offer two high resistive storage states, and thus, parasitic sneak currents are efficiently avoided. However, until now the CRS-based logic-in-memory approach was only shown to be able to perform basic Boolean logic operations using a single CRS cell. In this paper, we introduce two multi-bit adder schemes using the CRS-based logic-in-memory approach. We proof the concepts by means of SPICE simulations using a dynamical memristive device model of a ReRAM cell. Finally, we show the advantages of our novel adder concept in terms of step count and number of devices in comparison to a recently published adder approach, which applies the conventional ReRAM-based sequential logic concept introduced by Borghetti et al.",1410.2031v2 2014-10-13,Resistant Multiple Sparse Canonical Correlation,"Canonical Correlation Analysis (CCA) is a multivariate technique that takes two datasets and forms the most highly correlated possible pairs of linear combinations between them. Each subsequent pair of linear combinations is orthogonal to the preceding pair, meaning that new information is gleaned from each pair. By looking at the magnitude of coefficient values, we can find out which variables can be grouped together, thus better understanding multiple interactions that are otherwise difficult to compute or grasp intuitively. CCA appears to have quite powerful applications to high throughput data, as we can use it to discover, for example, relationships between gene expression and gene copy number variation. One of the biggest problems of CCA is that the number of variables (often upwards of 10,000) makes biological interpretation of linear combinations nearly impossible. To limit variable output, we have employed a method known as Sparse Canonical Correlation Analysis (SCCA), while adding estimation which is resistant to extreme observations or other types of deviant data. In this paper, we have demonstrated the success of resistant estimation in variable selection using SCCA. Additionally, we have used SCCA to find multiple canonical pairs for extended knowledge about the datasets at hand. Again, using resistant estimators provided more accurate estimates than standard estimators in the multiple canonical correlation setting. R code is available and documented at https://github.com/hardin47/rmscca.",1410.3355v2 2014-12-19,Magnetoresistance near a quantum critical point,"In metals near a quantum critical point, the electrical resistance is thought to be determined by the lifetime of the carriers of current, rather than the scattering from defects. The observation of $T$-linear resistivity suggests that the lifetime only depends on temperature, implying the vanishing of an intrinsic energy scale and the presence of a quantum critical point. Our data suggest that this concept extends to the magnetic field dependence of the resistivity in the unconventional superconductor BaFe$_2$(As$_{1-x}$P$_{x}$)$_2$ near its quantum critical point. We find that the lifetime depends on magnetic field in the same way as it depends on temperature, scaled by the ratio of two fundamental constants $\mu_B/k_B$. These measurements imply that high magnetic fields probe the same quantum dynamics that give rise to the $T$-linear resistivity, revealing a novel kind of magnetoresistance that does not depend on details of the Fermi surface, but rather on the balance of thermal and magnetic energy scales. This opens new opportunities for the investigation of transport near a quantum critical point by using magnetic fields to couple selectively to charge, spin and spatial anisotropies.",1412.6484v2 2015-08-14,Lattice Boltzmann model for resistive relativistic magnetohydrodynamics,"In this paper, we develop a lattice Boltzmann model for relativistic magnetohydrodynamics (MHD). Even though the model is derived for resistive MHD, it is shown that it is numerically robust even in the high conductivity (ideal MHD) limit. In order to validate the numerical method, test simulations are carried out for both ideal and resistive limits, namely the propagation of Alfv\'en waves in the ideal MHD and the evolution of current sheets in the resistive regime, where very good agreement is observed comparing to the analytical results. Additionally, two-dimensional magnetic reconnection driven by Kelvin-Helmholtz instability is studied and the effects of different parameters on the reconnection rate are investigated. It is shown that the density ratio has negligible effect on the magnetic reconnection rate, while an increase in shear velocity decreases the reconnection rate. Additionally, it is found that the reconnection rate is proportional to $\sigma^{-\frac{1}{2}}$, $\sigma$ being the conductivity, which is in agreement with the scaling law of the Sweet-Parker model. Finally, the numerical model is used to study the magnetic reconnection in a stellar flare. Three-dimensional simulation suggests that the reconnection between the background and flux rope magnetic lines in a stellar flare can take place as a result of a shear velocity in the photosphere.",1508.03452v1 2015-10-12,First in-beam studies of a Resistive-Plate WELL gaseous multiplier,"We present the results of the first in-beam studies of a medium size (10$\times$10 cm$^2$) Resistive-Plate WELL (RPWELL): a single-sided THGEM coupled to a pad anode through a resistive layer of high bulk resistivity ($\sim$10$^9 \Omega$cm). The 6.2~mm thick (excluding readout electronics) single-stage detector was studied with 150~GeV muons and pions. Signals were recorded from 1$\times$1 cm$^2$ square copper pads with APV25-SRS readout electronics. The single-element detector was operated in Ne\(5% $\mathrm{CH_{4}}$) at a gas gain of a few times 10$^4$, reaching 99$\%$ detection efficiency at average pad multiplicity of $\sim$1.2. Operation at particle fluxes up to $\sim$10$^4$ Hz/cm$^2$ resulted in $\sim$23$\%$ gain drop leading to $\sim$5$\%$ efficiency loss. The striking feature was the discharge-free operation, also in intense pion beams. These results pave the way towards robust, efficient large-scale detectors for applications requiring economic solutions at moderate spatial and energy resolutions.",1510.03116v2 2016-04-14,Magnetotransport of single crystalline YSb,"We report magnetic field dependent transport measurements on a single crystal of cubic YSb together with first principles calculations of its electronic structure. The transverse magnetoresistance does not saturate up to 9 T and attains a value of 75,000 % at 1.8 K. The Hall coefficient is electron-like at high temperature, changes sign to hole-like between 110 and 50 K, and again becomes electron-like below 50 K. First principles calculations show that YSb is a compensated semimetal with a qualitatively similar electronic structure to that of isostructural LaSb and LaBi, but with larger Fermi surface volume. The measured electron carrier density and Hall mobility calculated at 1.8 K, based on a single band approximation, are 6.5$\times10^{20}/$cm$^{3}$ and 6.2$\times10^{4}$cm$^{2}$/Vs, respectively. These values are comparable with those reported for LaBi and LaSb. Like LaBi and LaSb, YSb undergoes a magnetic field-induced metal-insulator-like transition below a characteristic temperature T$_{m}$, with resistivity saturation below 13 K. Thickness dependent electrical resistance measurements show a deviation of the resistance behavior from that expected for a normal metal; however, they do not unambiguously establish surface conduction as the mechanism for the resistivity plateau.",1604.04232v1 2017-02-14,A magnetic skyrmion as a non-linear resistive element - a potential building block for reservoir computing,"Inspired by the human brain, there is a strong effort to find alternative models of information processing capable of imitating the high energy efficiency of neuromorphic information processing. One possible realization of cognitive computing are reservoir computing networks. These networks are built out of non-linear resistive elements which are recursively connected. We propose that a skyrmion network embedded in frustrated magnetic films may provide a suitable physical implementation for reservoir computing applications. The significant key ingredient of such a network is a two-terminal device with non-linear voltage characteristics originating from single-layer magnetoresistive effects, like the anisotropic magnetoresistance or the recently discovered non-collinear magnetoresistance. The most basic element for a reservoir computing network built from ""skyrmion fabrics"" is a single skyrmion embedded in a ferromagnetic ribbon. In order to pave the way towards reservoir computing systems based on skyrmion fabrics, here we simulate and analyze i) the current flow through a single magnetic skyrmion due to the anisotropic magneto-resistive effect and ii) the combined physics of local pinning and the anisotropic magneto-resistive effect.",1702.04298v2 2017-06-15,MAGNUS: A new resistive MHD code with heat flow terms,"We present a new magnetohydrodynamic (MHD) code for the simulation of wave propagation in the solar atmosphere, under the effects of electrical resistivity, but not dominant, and heat transference in a uniform 3D grid. The code is based on the finite volume method combined with the HLLE and HLLC approximate Riemann solvers, which use different slope limiters like MINMOD, MC, and WENO5. In order to control the growth of the divergence of the magnetic field, due to numerical errors, we apply the Flux Constrained Transport method, which is described in detail to understand how the resistive terms are included in the algorithm. In our results, it is verified that this method preserves the divergence of the magnetic fields within the machine round-off error. For the validation of the accuracy and efficiency of the schemes implemented in the code, we present some numerical tests in 1D and 2D for the ideal MHD. Later, we show one test for the resistivity in a magnetic reconnection process and one for the thermal conduction, where the temperature is advected by the magnetic field lines. Moreover, we display two numerical problems associated with the MHD wave propagation. The first one corresponds to a 3D evolution of a vertical velocity pulse at the photosphere-transition-corona region, while the second one consists in a 2D simulation of a transverse velocity pulse in a coronal loop.",1706.05110v1 2018-02-06,Radiation resistant LGAD design,"In this paper, we report on the radiation resistance of 50-micron thick LGAD detectors manufactured at the Fondazione Bruno Kessler employing several different doping combinations of the gain layer. LGAD detectors with gain layer doping of Boron, Boron low-diffusion, Gallium, Carbonated Boron and Carbonated Gallium have been designed and successfully produced. These sensors have been exposed to neutron fluences up to $\phi_n \sim 3 \cdot 10^{16}\; n/cm^2$ and to proton fluences up to $\phi_p \sim 9\cdot10^{15}\; p/cm^2$ to test their radiation resistance. The experimental results show that Gallium-doped LGADs are more heavily affected by initial acceptor removal than Boron-doped LGAD, while the presence of Carbon reduces initial acceptor removal both for Gallium and Boron doping. Boron low-diffusion shows a higher radiation resistance than that of standard Boron implant, indicating a dependence of the initial acceptor removal mechanism upon the implant width. This study also demonstrates that proton irradiation is at least twice more effective in producing initial acceptor removal, making proton irradiation far more damaging than neutron irradiation.",1802.01745v4 2018-04-14,Non-resistive dissipative magnetohydrodynamics from the Boltzmann equation in the 14-moment approximation,"We derive the equations of motion of relativistic, non-resistive, second-order dissipative magnetohydrodynamics from the Boltzmann equation using the method of moments. We assume the fluid to be composed of a single type of point-like particles with vanishing dipole moment or spin, so that the fluid has vanishing magnetization and polarization. In a first approximation, we assume the fluid to be non-resistive, which allows to express the electric field in terms of the magnetic field. We derive equations of motion for the irreducible moments of the deviation of the single-particle distribution function from local thermodynamical equilibrium. We analyze the Navier-Stokes limit of these equations, reproducing previous results for the structure of the first-order transport coefficients. Finally, we truncate the system of equations for the irreducible moments using the 14-moment approximation, deriving the equations of motion of relativistic, non-resistive, second-order dissipative magnetohydrodynamics. We also give expressions for the new transport coefficients appearing due to the coupling of the magnetic field to the dissipative quantities.",1804.05210v2 2018-03-30,"Linearity Analysis of the Common Collector Amplifier, or Emitter Follower","A recently introduced Early modeling of transistors is applied to the study of the common collector amplifier (or emitter follower), an important type of electronic circuit typically employed as buffer, being characterized by near unit voltage gain, high input resistance, and low output resistance. The Early equivalent model is applied to derive a simple representation that is simple and yet capable of incorporating the transistor non-linearities implied by the Early effect. Mathematical expressions are obtained describing completely the circuit operation in terms of currents and voltages, allowing accurate estimation of the average voltage gain, total harmonic distortion (THD), and average input and output resistances. Prototypes of small signal silicon transistors of types NPN and PNP obtained in a previous work are used to discuss the respectively implied properties of the common collector transistor. In addition to confirming the importance of the trade-off of current gain for the desired properties, it is also shown that sub-optimal performance can be obtained in case the base and emitter resistances are not properly chosen. Even so, the limited current gain implied by real-world NPN and PNP small signal silicon devices implies some performance constraints. In particular, it has been observed that the THD tends to be larger for PNP devices than NPN counterparts with the same average current gain. The obtained results pave the way not only to complementary analytical studies, but also provide guidance for design and implementation of improved common collector configurations.",1805.02705v1 2018-11-23,Oxygen vacancies dynamics in redox-based interfaces: Tailoring the memristive response,"Redox-based memristive devices are among the alternatives for the next generation of non volatile memories, but also candidates to emulate the behavior of synapses in neuromorphic computing devices. It is nowadays well established that the motion of oxygen vacancies (OV) at the nanoscale is the key mechanism to reversibly switch metal/insulator/metal structures from insulating to conducting, i.e. to accomplish the resistive switching effect. The control of OV dynamics has a direct effect on the resistance changes, and therefore on different figures of memristive devices, such as switching speed, retention, endurance or energy consumption. Advances in this direction demand not only experimental techniques that allow for measurements of OV dynamics, but also of theoretical studies that shed light on the involved mechanisms. Along this goal, we analize the OV dynamics in redox interfaces formed when an oxidizable metallic electrode is in contact with the insulating oxide. We show how the transfer of OV can be manipulated by using different electrical stimuli protocols to optimize device figures such as the ON/OFF ratio or the energy dissipation linked to the writing process. Analytical expressions for attained resistance values, including the high and low resistance states are derived in terms of total transferred OV in a nanoscale region of the interface. Our predictions are validated with experiments performed in Ti/La$_{1/3}$Ca$_{2/3}$MnO$_{3}$ redox memristive devices.",1811.09528v1 2014-08-14,"Crystal growth and annealing study of fragile, non-bulk superconductivity in YFe$_2$Ge$_2$","We investigated the occurrence and nature of superconductivity in single crystals of YFe$_2$Ge$_2$ grown out of Sn flux by employing x-ray diffraction, electrical resistivity, and specific heat measurements. We found that the residual resistivity ratio (RRR) of single crystals can be greatly improved, reaching as high as $\sim$60, by decanting the crystals from the molten Sn at $\sim$350$^\circ$C and/or by annealing at temperatures between 550$^\circ$C and 600$^\circ$C. We found that samples with RRR $\gtrsim$ 34 showed resistive signatures of superconductivity with the onset of the superconducting transition $T_c\approx1.4$ K. RRR values vary between 35 and 65 with, on average, no systematic change in $T_c$ value, indicating that systematic changes in RRR do not lead to comparable changes in $T_c$. Specific heat measurements on samples that showed clear resistive signatures of a superconducting transition did not show any signature of a superconducting phase transition, which suggests that the superconductivity observed in this compound is either some sort of filamentary, strain stabilized superconductivity associated with small amounts of stressed YFe$_2$Ge$_2$ (perhaps at twin boundaries or dislocations) or is a second crystallographic phase present at levels below detection capability of conventional powder x-ray techniques.",1408.3319v1 2019-07-17,A Nanomagnetic Voltage-Tunable Correlation Generator between Two Random Bit Streams for Stochastic Computing,"Graphical probabilistic circuit models of stochastic computing are more powerful than the predominant deep learning models, but also have more demanding requirements. For example, they require ""programmable stochasticity"", e.g. generating two random binary bit streams with tunable amount of correlation between the corresponding bits in the two streams. Electronic implementation of such a system would call for several components leaving a large footprint on a chip and dissipating excessive amount of energy. Here, we show an elegant implementation with just two dipole-coupled magneto-tunneling junctions (MTJ), with magnetostrictive soft layers, fabricated on a piezoelectric film. The resistance states of the two MTJs (high or low) encode the bits in the two streams. The first MTJ is driven to a random resistance state via a current or voltage generating spin transfer torque and/or voltage controlled magnetic anisotropy, while the second MTJ's resistance state is determined solely by dipole coupling with the first. The effect of dipole coupling can be varied with local strain applied to the second MTJ with a local voltage (~0.2 V) and that varies the correlation between the resistance states of the two MTJs and hence between the bits in the two streams (from 0% to 100%). This paradigm can be extended to arbitrary number of bit streams.",1907.07532v1 2017-04-26,Identifying Similarities in Epileptic Patients for Drug Resistance Prediction,"Currently, approximately 30% of epileptic patients treated with antiepileptic drugs (AEDs) remain resistant to treatment (known as refractory patients). This project seeks to understand the underlying similarities in refractory patients vs. other epileptic patients, identify features contributing to drug resistance across underlying phenotypes for refractory patients, and develop predictive models for drug resistance in epileptic patients. In this study, epileptic patient data was examined to attempt to observe discernable similarities or differences in refractory patients (case) and other non-refractory patients (control) to map underlying mechanisms in causality. For the first part of the study, unsupervised algorithms such as Kmeans, Spectral Clustering, and Gaussian Mixture Models were used to examine patient features projected into a lower dimensional space. Results from this study showed a high degree of non-linearity in the underlying feature space. For the second part of this study, classification algorithms such as Logistic Regression, Gradient Boosted Decision Trees, and SVMs, were tested on the reduced-dimensionality features, with accuracy results of 0.83(+/-0.3) testing using 7 fold cross validation. Observations of test results indicate using a radial basis function kernel PCA to reduce features ingested by a Gradient Boosted Decision Tree Ensemble lead to gains in improved accuracy in mapping a binary decision to highly non-linear features collected from epileptic patients.",1704.08361v1 2019-06-24,Fully Dynamic Spectral Vertex Sparsifiers and Applications,"We study \emph{dynamic} algorithms for maintaining spectral vertex sparsifiers of graphs with respect to a set of terminals $T$ of our choice. Such objects preserve pairwise resistances, solutions to systems of linear equations, and energy of electrical flows between the terminals in $T$. We give a data structure that supports insertions and deletions of edges, and terminal additions, all in sublinear time. Our result is then applied to the following problems. (1) A data structure for maintaining solutions to Laplacian systems $\mathbf{L} \mathbf{x} = \mathbf{b}$, where $\mathbf{L}$ is the Laplacian matrix and $\mathbf{b}$ is a demand vector. For a bounded degree, unweighted graph, we support modifications to both $\mathbf{L}$ and $\mathbf{b}$ while providing access to $\epsilon$-approximations to the energy of routing an electrical flow with demand $\mathbf{b}$, as well as query access to entries of a vector $\tilde{\mathbf{x}}$ such that $\left\lVert \tilde{\mathbf{x}}-\mathbf{L}^{\dagger} \mathbf{b} \right\rVert_{\mathbf{L}} \leq \epsilon \left\lVert \mathbf{L}^{\dagger} \mathbf{b} \right\rVert_{\mathbf{L}}$ in $\tilde{O}(n^{11/12}\epsilon^{-5})$ expected amortized update and query time. (2) A data structure for maintaining All-Pairs Effective Resistance. For an intermixed sequence of edge insertions, deletions, and resistance queries, our data structure returns $(1 \pm \epsilon)$-approximation to all the resistance queries against an oblivious adversary with high probability. Its expected amortized update and query times are $\tilde{O}(\min(m^{3/4},n^{5/6} \epsilon^{-2}) \epsilon^{-4})$ on an unweighted graph, and $\tilde{O}(n^{5/6}\epsilon^{-6})$ on weighted graphs. These results represent the first data structures for maintaining key primitives from the Laplacian paradigm for graph algorithms in sublinear time without assumptions on the underlying graph topologies.",1906.10530v1 2019-11-18,Comparison of screening for methicillin-resistant Staphylococcus aureus (MRSA) at hospital admission and discharge,"Methicillin-resistant Staphylococcus aureus (MRSA) is a significant contributor to the growing concern of antibiotic resistant bacteria, especially given its stubborn persistence in hospitals and other health care facility settings. In combination with this characteristic of S. aureus (colloquially referred to as staph), MRSA presents an additional barrier to treatment and is now believed to have colonized two of every 100 people worldwide. According to the CDC, MRSA prevalence sits as high as 25-50% in countries such as the United Kingdom and the United States. Given the resistant nature of staph as well as its capability of evolving to compensate antibiotic treatment, controlling MRSA levels is more a matter of precautionary and defensive measures. This study examines the method of ""search and isolation,"" which seeks to isolate MRSA positive patients in a hospital so as to decrease infection potential. Although this strategy is straightforward, the question of just whom to screen is of practical importance. We compare screening at admission to screening at discharge. To do this, we develop a mathematical model and use simulations to determine MRSA endemic levels in a hospital with either control measure implemented. We found that screening at discharge was the more effective method in controlling MRSA endemicity, but at the cost of a greater number of isolated patients.",1911.07711v1 2020-07-02,Bloch-Grüneisen temperature and universal scaling of normalized resistivity in doped graphene revisited,"In this work, we resolved some controversial issues on the Bloch-Gr\""{u}neisen (BG) temperature in doped graphene via analytical and numerical calculations based on full inelastic electron-acoustic-phonon (EAP) scattering rate and various approximation schemes. Analytic results for BG temperature obtained by semi-inelastic (SI) approximation (which gives scattering rates in excellent agreement with the full inelastic scattering rates) are compared with those obtained by quasi-elastic (QE) approximation and the commonly adopted value of $\Theta^{LA}_{F} = 2\hbar v_{LA} k_F/k_B$. It is found that the commonly adopted BG temperature in graphene ($\Theta^{LA}_{F}$) is about 5 times larger than the value obtained by the QE approximation and about 2.5 times larger than that by the SI approximation, when using the crossing-point temperature where low-temperature and high-temperature limits of the resistivity meet. The corrected analytic relation based on SI approximation agrees extremely well with the transition temperatures determined by fitting the the low- and high-$T$ behavior of available experimental data of graphene's resistivity. We also introduce a way to determine the BG temperature including the full inelastic EAP scattering rate and the deviation of electron energy from the chemical potential ($\mu$) numerically by finding the maximum of $\partial \rho(\mu,T)/\partial T$. Using the analytic expression of $\Theta_{BG,1}$ we can prove that the normalized resistivity defined as $R_{1}=\rho(\mu,T)/\rho(\mu,\Theta_{BG,1})$ plotted as a function of $(T/\Theta_{BG,1})$ is independent of the carrier density. Applying our results to previous experimental data extracted shows a universal scaling behavior, which is different from previous studies.",2007.00839v1 2020-11-16,Transition region from turbulent to dead zone in protoplanetary disks: local shearing box simulations,"The dynamical evolution of protoplanetary disks is of key interest for building a comprehensive theory of planet formation and to explain the observational properties of these objects. Using the magnetohydrodynamics code Athena++, with an isothermal shearing box setup, we study the boundary between the active and dead zone, where the accretion rate changes and mass can accumulate. We quantify how the turbulence level is affected by the presence of a non uniform ohmic resistivity in the radial-x direction that leads to a region of inhibited turbulence (or dead zone). Comparing the turbulent activity to that of ideal simulations, the turbulence inhibited area shows density fluctuations and magnetic activity at its boundaries, driven by energy injection from the active (ideal) zone boundaries. We find magnetic dissipation to be significantly stronger in the ideal regions, and the turbulence penetration through the boundary of the dead zone is determined by the value of the resistivity itself, through the ohmic dissipation process, though the thickness of the transition does not play a significant role in changing the dissipation. We investigate the 1D spectra along the shearing direction: magnetic spectra appear flat at large scales both in ideal as well as resistive simulations, though a Kolmogorov scaling over more than one decade persists in the dead zone, suggesting the turbulent cascade is determined by the hydrodynamics of the system: MRI dynamo action is inhibited where sufficiently high resistivity is present.",2011.08219v1 2021-10-21,E-DPNCT: An Enhanced Attack Resilient Differential Privacy Model For Smart Grids Using Split Noise Cancellation,"High frequency reporting of energy consumption data in smart grids can be used to infer sensitive information regarding the consumer's life style and poses serious security and privacy threats. Differential privacy (DP) based privacy models for smart grids ensure privacy when analysing energy consumption data for billing and load monitoring. However, DP models for smart grids are vulnerable to collusion attack where an adversary colludes with malicious smart meters and un-trusted aggregator in order to get private information from other smart meters. We first show the vulnerability of DP based privacy model for smart grids against collusion attacks to establish the need of a collusion resistant model privacy model. Then, we propose an Enhanced Differential Private Noise Cancellation Model for Load Monitoring and Billing for Smart Meters (E-DPNCT) which not only provides resistance against collusion attacks but also protects the privacy of the smart grid data while providing accurate billing and load monitoring. We use differential privacy with a split noise cancellation protocol with multiple master smart meters (MSMs) to achieve colluison resistance. We did extensive comparison of our E-DPNCT model with state of the art attack resistant privacy preserving models such as EPIC for collusion attack. We simulate our E-DPNCT model with real time data which shows significant improvement in privacy attack scenarios. Further, we analyze the impact of selecting different sensitivity parameters for calibrating DP noise over the privacy of customer electricity profile and accuracy of electricity data aggregation such as load monitoring and billing.",2110.11091v4 2022-05-10,Disorder-enhanced effective masses and deviations from Matthiessen's rule in PdCoO$_2$ thin films,"The observation of hydrodynamic transport in the metallic delafossite PdCoO$_2$ has increased interest in this family of highly conductive oxides, but experimental studies so far have mostly been confined to bulk crystals. In this work, the development of high-quality thin films of PdCoO$_2$ has enabled a thorough study of the conductivity as a function of film thickness using both dc transport and time-domain THz spectroscopy. With increasing film thickness from 12 nm to 102 nm, the residual resistivity decreases and we observe a large deviation from Matthiessen's rule (DMR) in the temperature dependence of the resistivity. We find that the complex THz conductivity is well fit by a single Drude term. We fit the data to extract the spectral weight and scattering rate simultaneously. The temperature dependence of the Drude scattering rate is found to be nearly independent of the residual resistivity and cannot be the primary mechanism for the observed DMR. Rather, we observe large changes in the spectral weight as a function of disorder, changing by a factor of 1.5 from the most disordered to least disordered films. We believe this corresponds to a mass enhancement of $\geq 2$ times the value of the bulk effective mass which increases with residual disorder. This suggests that the mechanism behind the DMR observed in dc resistivity is primarily driven by changes in the electron mass. We discuss the possible origins of this behavior including the possibility of disorder-enhanced electron-phonon scattering, which can be systematically tuned by film thickness.",2205.05006v2 2022-08-05,Hall effect in Poiseuille flow of two-dimensional electron fluid,"The hydrodynamic regime of charge transport has been recently realized in high-quality conductors. In the hydrodynamic as well as in the Ohmic regimes the main part of the Hall resistance of a long sample is determined by the balance between the Lorentz force and the electric force, acting on conduction electrons. Experimentally observed deviations of the Hall resistance in hydrodynamic samples from such the ''standard'' value are usually associated with the Hall viscosity term in the Navier-Stokes equation. In this work we theoretically study the Hall effect in a Poiseuille flow of a two-dimensional electron fluid. We show that the near-edge semiballistic layers with the width of the order of the inter-particle mean free path, which inevitably appear near sample edges, give the contribution to the Hall resistance which is comparable with the bulk contribution from the Hall viscosity. In this way, the measured deviations of the Hall resistance from the ''standard'' one in hydrodynamic samples by the usual contact techniques should be associated with both the Hall viscosity in the bulk and the semiballistic effects in the near-edge layers",2208.03032v1 2022-10-28,Lattice effects on the physical properties of half doped perovskite ruthenates,"We investigate the unusual phase transitions in SrRuO$_{3}$ and Sr$_{0.5}$Ca$_{0.5}$Ru$_{1-x}$Cr$_{x}$O$_{3}$ (x=0,0.05 and 0.1) employing x-ray diffraction, resistivity, magnetic studies and x-ray photoemission spectroscopy. Our results show the compounds undergo crossover from $itinerant$ ferromagnetism to $localised$ ferromagnetism. The combined studies suggests Ru and Cr to be in 4+ valence state. A Griffith phase and an enhancement in Curie temperature (Tc) from 38 K to 107 K is observed with Cr doping. A shift in the chemical potential towards the valence band is observed with Cr doping. In the metallic samples, interestingly, a direct link between the resistivity and orthorhombic strain is observed. Detailed studies in this direction will be helpful to understand the nature of interactions and hence manoeuvre its properties. In the non metallic samples, the resistivity is mainly governed by disorder and electron-electron correlation effects. The value of the resistivity for the 5% Cr doped sample suggests semi metallic behaviour. Understanding its nature in detail using electron spectroscopic techniques could unravel the possibility of its utility in high mobility transistors at room temperature and its combined property with ferromagnetism will be helpful in making spintronic devices.",2210.16036v1 2022-12-05,DeAR: A Deep-learning-based Audio Re-recording Resilient Watermarking,"Audio watermarking is widely used for leaking source tracing. The robustness of the watermark determines the traceability of the algorithm. With the development of digital technology, audio re-recording (AR) has become an efficient and covert means to steal secrets. AR process could drastically destroy the watermark signal while preserving the original information. This puts forward a new requirement for audio watermarking at this stage, that is, to be robust to AR distortions. Unfortunately, none of the existing algorithms can effectively resist AR attacks due to the complexity of the AR process. To address this limitation, this paper proposes DeAR, a deep-learning-based audio re-recording resistant watermarking. Inspired by DNN-based image watermarking, we pioneer a deep learning framework for audio carriers, based on which the watermark signal can be effectively embedded and extracted. Meanwhile, in order to resist the AR attack, we delicately analyze the distortions that occurred in the AR process and design the corresponding distortion layer to cooperate with the proposed watermarking framework. Extensive experiments show that the proposed algorithm can resist not only common electronic channel distortions but also AR distortions. Under the premise of high-quality embedding (SNR=25.86dB), in the case of a common re-recording distance (20cm), the algorithm can effectively achieve an average bit recovery accuracy of 98.55%.",2212.02339v4 2023-04-18,Characterization of a Superconducting Microstrip Single-Photon Detector Shunted with an External Resistor,"A superconducting microstrip single-photon detector (SMSPD) generally requires a shunt resistor to avoid latching, caused by its high current-carrying capacity and low kinetic inductance. Here, the effect of the shunt resistor on the behaviors of microbridge SMSPDs was investigated. We analyzed the change in equivalent switching current at different shunt resistances in two ways and determined the operating current range using intrinsic dark count rate (iDCR) curves. We observed that the reduction in shunt resistance can increase the operating current range, which helps to improve the internal detection efficiency (IDE) and reduce the iDCR. However, the reduction in the shunt resistance can reduce the pulse amplitude and increase the pulse decay time, which can degrade the timing jitter and count rate performance of the SMSPD. The trends of the experimental results can be qualitatively reproduced using a circuit model for an SMSPD with a shunt resistor, which provides useful information for the selection of shunt resistors. Furthermore, we report the improved detection performance of a helium-ion-irradiated SMSPD shunted with a small resistance of 5.2 {\Omega}. We observed a weak IDE saturation with a bias current at a wavelength up to 2000 nm and a nonlinear relation between detection current and photon energy.",2304.08762v1 2023-05-18,Fabrication of Al/AlOx/Al junctions with high uniformity and stability on sapphire substrates,"Tantalum and aluminum on sapphire are widely used platforms for qubits of long coherent time. As quantum chips scale up, the number of Josephson junctions on Sapphire increases. Thus, both the uniformity and stability of the junctions are crucial to quantum devices, such as scalable superconducting quantum computer circuit, and quantum-limited amplifiers. By optimizing the fabrication process, especially, the conductive layer during the electron beam lithography process, Al/AlOx/Al junctions of sizes ranging from 0.0169 to 0.04 {\mu}m2 on sapphire substrates were prepared. The relative standard deviation of room temperature resistances (RN) of these junctions is better than 1.7% on 15 mmx15 mm chips, and better than 2.66% on 2 inch wafers, which is the highest uniformity on sapphire substrates has been reported. The junctions are robust and stable in resistances as temperature changes. The resistances increase by the ratio of 9.73% relative to RN as the temperature ramp down to 4K, and restore their initial values in the reverse process as the temperature ramps back to RT. After being stored in a nitrogen cabinet for 100 days, the resistance of the junctions changed by1.16% in average. The demonstration of uniform and stable Josephson junctions in large area paves the way for the fabrication of superconducting chip of hundreds of qubits on sapphire substrates.",2305.10956v2 2023-06-21,Coherent states and their superpositions (cat states) in microwave-induced resistance oscillations,"We report a novel theoretical approach on the microwave-induced resistance oscillations based on the coherent states of the quantum harmonic oscillator. We first obtain an expression for the coherent states of driven-quantum harmonic oscillators that are used, in the model of microwaveinduced electron orbits, to calculate magnetoresistance under radiation. Thus, we find that the principle of minimum uncertainty of coherent states, involving time and energy, is at the heart of photo-oscillations and zero resistance states. Accordingly, we are able to explain important experimental evidence of this remarkable effect. Such as the physical origin of oscillations, their periodicity with the inverse of the magnetic field, their peculiar minima and maxima positions and the existence of zero resistance states. We apply our theory to the case of ultra-high mobility samples where we appeal to the principle of quantum superposition of coherent states and obtain that Schrodinger cat states (even and odd coherent states) are key to explain magnetoresistance at these extreme mobilities. With them we explain the, experimentally obtained, magnetoresistance resonance peak shift to a magnetic field where the cyclotron frequency equals half the radiation frequency. This effect is similar to the one described in quantum optics as a second harmonic generation process. We also explain the magnetoresistance collapse, that take place in the dark and with light. This effect is known as giant negative magnetoresistance. We generalize our results to study the case of a three-component or triangular Schrodinger cat state.",2306.12160v1 2023-08-28,Research on the Influence of Underwater Environment on the Dynamic Performance of the Mechanical Leg of a Deep-sea Crawling and Swimming Robot,"The performance of underwater crawling and adjustment of the body posture for underwater manipulating of the deep-sea crawling and swimming robot (DCSR) is directly influenced by the dynamic performance of the underwater mechanical legs (UWML), as it serves as the executive mechanism of the DCSR. Compared with the mechanical legs of legged robots working on land, the UWML of the DCSR not only possesses the characteristics of the land used mechanical legs, but is also affected by the influence of the deep-sea underwater working environment (i.e., the hydrodynamic force, viscous resistance and dynamic seal resistance). To reduce these influence, firstly, the hydrodynamic force of the UWML were researched based on theory and experiment, and the hydrodynamic model was established with the fitted hydrodynamic parameters. Secondly, the oil viscous resistance and the dynamic seal resistance were studied experimentally, and the change laws of both with respect to the joint speed and the ambient pressure (depth of operation) were obtained. The results provide a basis for the subsequent research on the structure optimization and high performance control of the UWML and DCSR.",2308.14393v1 2023-11-17,Current manipulation of Giant tunneling altermagnetic resistance in collinear Antiferromagnetic RuO2/MgO/RuO2 sandwich structure,"As an emerging non-volatile memory technology, magnetic random access memory (MRAM) has key features and advantages including non-volatility, high speed, endurance, low power consumption and radiation tolerance. Conventional MRAM utilizes magnetic tunnel junctions (MTJs), which consist of two ferromagnetic layers separated by an insulating tunnel barrier. The orientation of the magnetic layers represents the binary data (0 or 1), and electrical resistance changes depending on the relative orientation of these magnetic layers. Despite these advancements, the quest for a swifter, more stable magneto-resistive random-access memory paradigm persists. In this vein, we present a groundbreaking development: room-temperature antiferromagnetic tunnel junctions devoid of any net magnetic moment. Over 200% tunneling altermagnetic resistance (TAR) ratio was measured at RuO2 (110)/MgO/RuO2 (110)/W structure, which is achieved by changing the antiferromagnetic Neel vector of RuO2 with an ultralow current density 2 MA*cm-2.",2311.10288v2 2024-02-09,Wellposedness of the electron MHD without resistivity for large perturbations of the uniform magnetic field,"We prove the local wellposedness of the Cauchy problems for the electron magnetohydrodynamics equations (E-MHD) without resistivity for possibly large perturbations of nonzero uniform magnetic fields. While the local wellposedness problem for (E-MHD) has been extensively studied in the presence of resistivity (which provides dissipative effects), this seems to be the first such result without resistivity. (E-MHD) is a fluid description of plasma in small scales where the motion of electrons relative to ions is significant. Mathematically, it is a quasilinear dispersive equation with nondegenerate but nonelliptic second-order principal term. Our result significantly improves upon the straightforward adaptation of the classical work of Kenig--Ponce--Rolvung--Vega on the quasilinear ultrahyperbolic Schr\""odinger equations, as the regularity and decay assumptions on the initial data are greatly weakened to the level analogous to the recent work of Marzuola--Metcalfe--Tataru in the case of elliptic principal term. A key ingredient of our proof is a simple observation about the relationship between the size of a symbol and the operator norm of its quantization as a pseudodifferential operator when restricted to high frequencies. This allows us to localize the (non-classical) pseudodifferential renormalization operator considered by Kenig--Ponce--Rolvung--Vega, and produce instead a classical pseudodifferential renormalization operator. We furthermore incorporate the function space framework of Marzuola--Metcalfe--Tataru to the present case of nonelliptic principal term.",2402.06278v1 2024-03-21,Aging suppression in Multistrip Multigap Resistive Plate Chambers for high counting rate experiments,"A long term operation of Multi-Strip Multi-Gap Resistive Plate Chambers (MSMGRPC) with gas mixtures based on C2H2F4 and SF6 leads to aging effects, observed as depositions on the surface of the resistive electrodes. Moreover, enhanced depositions and higher noise rates were evidenced around the nylon spacers used for defining the gas gaps between the resistive electrodes. The aging effects are reflected in an increase of the dark current and dark counting rate, with negative impact on the long term performance of the chamber and data volume in a free running readout mode operation. MSMGRPC prototypes designed with a direct gas flow through the gas gaps and minimization of the number of spacers in the active area were developed as mitigation solution. Prototypes with this new design and different granularities were assembled using fishing line as spacers and investigated for aging effects. Although a significant reduction in the dark current and dark counting rate was evidenced, dark counting rate localized around the fishing line spacers remains. In this paper, a new generation of direct flow chambers based on discrete spacers is presented. The results of their aging investigations show that, even at lower gas flows, the aging effects become negligible.",2403.14190v1 2006-03-20,Unusual metamagnetism in CeIrIn$_5$,"We report a high field investigation (up to 45 T) of the metamagnetic transition in CeIrIn$_5$ with resistivity and de-Haas-van-Alphen (dHvA) effect measurements in the temperature range 0.03-1 K. As the magnetic field is increased the resistivity increases, reaches a maximum at the metamagnetic critical field, and falls precipitously for fields just above the transition, while the amplitude of all measurable dHvA frequencies are significantly attenuated near the metamagnetic critical field. However, the dHvA frequencies and cyclotron masses are not substantially altered by the transition. In the low field state, the resistivity is observed to increase toward low temperatures in a singular fashion, a behavior that is rapidly suppressed above the transition. Instead, in the high field state, the resistivity monotonically increases with temperature with a dependence that is more singular than the iconic Fermi-liquid, temperature-squared, behavior. Both the damping of the dHvA amplitudes and the increased resistivity near the metamagnetic critical field indicate an increased scattering rate for charge carriers consistent with critical fluctuation scattering in proximity to a phase transition. The dHvA amplitudes do not uniformly recover above the critical field, with some hole-like orbits being entirely suppressed at high fields. These changes, taken as a whole, suggest that the metamagnetic transition in CeIrIn$_5$ is associated with the polarization and localization of the heaviest of quasiparticles on the hole-like Fermi surface.",0603490v2 2022-11-10,"T-linear resistivity, optical conductivity and Planckian transport for a holographic local quantum critical metal in a periodic potential","High $T_c$ cuprate strange metals are noted for a DC-resistivity that scales linearly with $T$ from the onset of superconductivity to the crystal melting temperature, indicative of a Planckian dissipation life time $\tau_{\hbar}\simeq \hbar /(k_B T)$. At the same time, the optical conductivity ceases to be of Drude form at high temperatures, suggesting a change of the underlying dynamics that surprisingly leaves the $T$-linear DC-resistivity unaffected. We use the AdS/CFT correspondence that describes strongly coupled, densely entangled metals to study DC thermo-electrical transport and the optical conductivities of the local quantum critical Gubser-Rocha holographic strange metal in the presence of a lattice potential, a prime candidate to compare with experiment. We find that the DC-resistivity is linear in $T$ at low temperatures for a range of lattice strengths and wavevectors, even as it transitions between different dissipative regimes. At weak lattice potential the optical conductivity evolves with increasing temperature from a Drude form to a bad-metal characterized by a mid-IR resonance without changing the DC transport, similar to that seen in cuprate strange metals. This mid-IR peak and its temperature evolution can be understood as a consequence of Umklapp hydrodynamics: hydrodynamic perturbations are Bloch modes in the presence of a lattice. At strong lattice potential an incoherent metal is realized instead where momentum conservation no longer plays a role in transport. In this regime the thermal diffusivity can be explained by Planckian dissipation originating in universal microscopic chaos, similar to holographic metals with strong homogeneous momentum relaxation. The charge diffusivity does not submit to this chaos explanation, even though the continuing linear-in-$T$ DC resistivity saturates to an apparent universal slope, numerically equal to a Planckian rate.",2211.05492v2 1998-05-20,A phenomenological model for magnetoresistance in granular polycrystalline colossal magnetoresistive materials: the role of spin polarised tunnelling at the grain boundaries,"It has been observed that in bulk and polycrystalline thin films of collossal magnetoresistive (CMR) materials the magnetoresistance follows a different behaviour compared to single crystals or single crystalline films below the ferromagnetic transition temperature Tc. In this paper we develop a phenomenological model to explain the magnetic field dependence of resistance in granular CMR materials taking into account the spin polarised tunnelling at the grain boundaries. The model has been fitted to two systems, namely, La0.55Ho0.15Sr0.3MnO3 and La1.8Y0.5Ca0.7Mn2O7. From the fitted result we have separated out, in La0.55Ho0.15Sr0.3MnO3, the intrinsic contribution from the intergranular contribution to the magnetoresistance coming from spin polarised tunnelling at the grain boundaries. It is observed that the temperature dependence of the intrinsic contribution to the magnetoresistance in La0.55Ho0.15Sr0.3MnO3 follows the prediction of double exchange model for all values of field.",9805258v1 2000-11-21,Anomalous NMR Spin-Lattice Relaxation in SrB_{6} and Ca_{1-x}La_{x}B_{6},"We report the results of {11}B nuclear magnetic resonance (NMR) measurements of SrB_{6} and Ca_{0.995}La_{0.05}B_{6} below room temperature. Although the electrical resistivities of these two materials differ substantially, their {11}B-NMR responses exhibit some strikingly common features. Both materials exhibit ferromagnetic order, but their {11}B-NMR spectra reveal very small hyperfine fields at the Boron sites. The spin lattice relaxation T_{1}^{-1} varies considerably with external field but changes with temperature only below a few K. We discuss these unusual results by considering various different scenarios for the electronic structure of these materials.",0011352v2 2004-07-17,Magneto - transport characterization of Dy123 monodomain superconductors,"The following report considers textured materials of the DyBa2Cu3O7 type seeded with a Nd123 seed as initiator. They are grown with an excess 20% Dy211 phase on a Dy2O3 substrate. We report chemical characterizations, electrical resistivity, thermoelectric power and thermal conductivity over a broad temperature range as a function of an applied magnetic field up to 6 T. We show that specific features appear on the magneto thermal transport properties different in these materials from those found in single crystals and polycrystalline samples. We propose that two vortex regimes can be distinguished in the mixed phase, - due to the intrinsic microstructure. We calculate the viscosity, entropy and figure of merit of the samples.",0407463v1 2007-01-09,Pressure Study of Superconductivity and Magnetism in Pure and Rh-Doped RuSr2GdCu2O8 Materials,"A hydrostatic pressure study was made on pure and Rh-doped specimens of the superconducting ferromagnetic compounds Ru1-xRhxSr2GdCu2O8 (x = 0-0.15) by means of measurement of electrical resistivity vs temperature, in pressures up to 2 GPa. Partial substitution of Rh for Ru decreases the magnetization of the material, lowers both the magnetic ordering temperature Tm, and the superconducting transition temperature Tc, and promotes granularity. The effect of pressure for all compositions is an increase in both the intra- and intergranular superconductivity transition temperatures, Tc and Tp respectively, as well as Tm. The rate of change of each transition temperature with pressure first drops for Rh concentrations near 5%, increasing latter for higher concentrations. While the rate of increase of Tc with pressure for all compositions is 2-3 times lower than in YBCO materials, the simultaneous increase of Tc and Tm with pressure could support the notion of competition between superconductivity and ferromagnetism in these materials. The effect of pressure on the weak-links was a significant improvement of inter-granular connectivity.",0701183v1 2007-04-25,Studies of the temperature and frequency dependent impedance of an electroceramic functional oxide thermistor,"The charge transport mechanism and the macroscopic dielectric constant in polycrystalline device materials commonly exhibit several components such as electrode-sample interface, grain boundary and bulk contributions. In order to gain precise understanding of the functionality of polycrystalline electroceramic device materials it is essential to deconvolute these contributions. The paradigm of functional thermistor ceramics based on thick film spinel manganates has been studied by temperature dependent alternating current impedance spectroscopy. Three typical relaxation phenomena were detected, which all showed a separated temperature dependence of resistivity consistent with thermally activated charge transport. The dominating grain boundary and the interface contributions exhibited distinctively different capacitance allowing clear identification. The composite nature of the dielectric properties in polycrystalline functional ceramics was emphasized, and impedance spectroscopy was shown to be a powerful tool to account for and model such behaviour.",0704.3378v1 2007-07-17,Gate-induced insulating state in bilayer graphene devices,"The potential of graphene-based materials consisting of one or a few layers of graphite for integrated electronics originates from the large room-temperature carrier mobility in these systems (approx. 10,000 cm2/Vs). However, the realization of electronic devices such as field-effect transistors will require controlling and even switching off the electrical conductivity by means of gate electrodes, which is made difficult by the absence of a bandgap in the intrinsic material. Here, we demonstrate the controlled induction of an insulating state - with large suppression of the conductivity - in bilayer graphene, by using a double-gate device configuration that allows an electric field to be applied perpendicular to the plane. The dependence of the resistance on temperature and electric field, and the absence of any effect in a single-layer device, strongly suggest that the gate-induced insulating state originates from the recently predicted opening of a bandgap between valence and conduction bands.",0707.2487v2 2009-05-12,Large magnetic entropy change near room temperature in antipervoskite SnCMn3,"We report the observation of large magnetocaloric effect near room temperature in antipervoskite SnCMn3. The maximal magnetic entropy change at the first-order ferrimagnetic-paramagnetic transition temperature (TC 279 K) is about 80.69mJ/cm3 K and 133mJ/cm3 K under the magnetic field of 20 kOe and 48 kOe, respectively. These values are close to those of typical magnetocaloric materials. The large magnetocaloric effect is associated with the sharp change of lattice, resistivity and magnetization in the vicinity of TC. Through the measurements of Seebeck coefficient and normal Hall effect, the title system is found to undergo a reconstruction of electronic structure at TC. Considering its low-cost and innocuous raw materials, Mn-based antiperovskite compounds are suggested to be appropriate for pursuing new materials with larger magnetocaloric effect.",0905.1773v1 2009-06-28,Partial Kekule Ordering of Adatoms on Graphene,"Electronic and transport properties of Graphene, a one-atom thick crystalline material, are sensitive to the presence of atoms adsorbed on its surface. An ensemble of randomly positioned adatoms, each serving as a scattering center, leads to the Bolzmann-Drude diffusion of charge determining the resistivity of the material. An important question, however, is whether the distribution of adatoms is always genuinely random. In this Article we demonstrate that a dilute adatoms on graphene may have a tendency towards a spatially correlated state with a hidden Kekule mosaic order. This effect emerges from the interaction between the adatoms mediated by the Friedel oscillations of the electron density in graphene. The onset of the ordered state, as the system is cooled below the critical temperature, is accompanied by the opening of a gap in the electronic spectrum of the material, dramatically changing its transport properties.",0906.5174v1 2012-02-13,Nanostructured antimony tin oxide synthesized via chemical precipitation method: its characterization and application in humidity sensing,"In present investigation we report the synthesis of antimony tin oxide nanoparticles via chemical precipitation method. The synthesized material was characterized using X-ray diffractometer, Scanning Electron Microscope, UV-visible absorption spectroscopy. XRD shows the crystalline nature of the synthesized material and the crystallite size was estimated by using Debye-Scherer equation and its minimum value was 3 nm. Pelletization of synthesized material was done using hydraulic press machine under uniform pressure of 616 MPa. Then the pellets were annealed at 200, 400 and 600{\deg}C. Further each pellet was put in humidity sensing chamber and corresponding variations in resistance with relative humidity (%RH) were measured. The average sensitivity was calculated by taking the average of all sensitivities ranging from 10 to 90% RH. The average sensitivity of the pellet annealed at 600{\deg}C was best among all the sensing pellets and was 2.18 K{\Omega}/%RH. Results were reproducible {\pm}84% after 2 months.",1205.2336v1 2012-02-13,Effect of nanostructured zinc oxide additives on the humidity and temperature sensing properties of cuprous oxide,"Present paper reports the effect of ZnO additives on humidity and temperature sensing properties of cuprous oxide. The cuprous oxide powder was mixed with 10% and 25% ZnO by weight and these samples were pelletized by using hydraulic pressing machine. The sensing materials were also investigated by Scanning Electron Microscope (SEM) and X-ray Diffraction (XRD). SEM images show morphology and porosity of material. The average particles size of cuprous oxide was found to be 1.2 micron. The sheet like structures of ZnO is evident in micrographs. From XRD all peaks are well identified and crystallite size for defferent peaks has also been calculated. The pellets of sensing materials were subjected to annealing at temperatures 200, 400 and 600 degrees C respectively and were exposed to humidity and temperature variations. Electrical resistances of pellets were found to vary with humidity and temperature and were recorded. The sensitivity of sensors at various temperature and humidity levels was calculated.",1205.2707v1 2012-05-29,"Transport Properties of Ni, Co, Fe, Mn Doped Cu0.01Bi2Te2.7Se0.3 for Thermoelectric Device Applications","Bi2Te3 based thermoelectric devices typically use a nickel layer as a diffusion barrier to block the diffusion of solder or copper atoms from the electrode into the thermoelectric material. Previous studies have shown degradation in the efficiency of these thermoelectric devices may be due to the diffusion of the barrier layer into the thermoelectric material. In this work Ni, Co, Fe, and Mn are intentionally doped into Cu0.01Bi2Te2.7Se0.3 in order to understand their effects on the thermoelectric material. Thermoelectric transport properties including the Seebeck coefficient, thermal conductivity, electrical resistivity, carrier concentration, and carrier mobility of Cu0.01Bi2Te2.7Se0.3 doped with 2 atomic percent M (M=Ni, Co, Fe, Mn) as Cu0.01Bi2Te2.7Se0.3M0.02, are studied in a temperature range of 5-525 K.",1205.6377v1 2012-07-04,Colossal Magnetoresistance in the Mn2+ Oxypnictides NdMnAsO1-xFx,"Colossal magnetoresistance (CMR) is a rare phenomenon in which the electronic resistivity of a material can be decreased by orders of magnitude upon application of a magnetic field. Such an effect could be the basis of the next generation of magnetic memory devices. Here we report CMR in the antiferromagnetic oxypnictide NdMnAsO1-xFx as a result of competition between an antiferromagnetic insulating phase with strong electron correlations and a paramagnetic semiconductor upon application of a magnetic field. The discovery of CMR in antiferromagnetic Mn2+ oxypnictide materials could open up an array of materials for further investigation and optimisation for technological applications.",1207.0958v1 2013-10-28,The d-p band-inversion topological insulator in bismuth-based skutterudites,"Skutterudites, a class of materials with cage-like crystal structure which have received considerable research interest in recent years, are the breeding ground of several unusual phenomena such as heavy fermion superconductivity, exciton-mediated superconducting state and Weyl fermions. Here, we predict a new topological insulator in bismuth-based skutterudites, in which the bands involved in the topological band-inversion process are d- and p-orbitals, which is distinctive with usual topological insulators, for instance in Bi2Se3 and BiTeI the bands involved in the topological band-inversion process are only p-orbitals. Due to the present of large d-electronic states, the electronic interaction in this topological insulator is much stronger than that in other conventional topological insulators. The stability of the new material is verified by binding energy calculation, phonon modes analysis, and the finite temperature molecular dynamics simulations. This new material can provide nearly zero-resistivity signal current for devices and is expected to be applied in spintronics devices.",1310.7413v2 2015-05-21,Ferromagnetism in Cr-doped topological insulator TlSbTe2,"We have synthesized a new ferromagnetic topological insulator by doping Cr to the ternary topological-insulator material TlSbTe2. Single crystals of Tl_{1-x}Cr_{x}SbTe2 were grown by a melting method and it was found that Cr can be incorporated into the TlSbTe2 matrix only within the solubility limit of about 1%. The Curie temperature \theta_c was found to increase with the Cr content but remained relatively low, with the maximum value of about 4 K. The easy axis was identified to be the c-axis and the saturation moment was 2.8 \mu_B (Bohr magneton) at 1.8 K. The in-plane resistivity of all the samples studied showed metallic behavior with p-type carriers. Shubnikov-de Hass (SdH) oscillations were observed in samples with the Cr-doping level of up to 0.76%. We also tried to induce ferromagnetism in TlBiTe2 by doping Cr, but no ferromagnetism was observed in Cr-doped TlBiTe2 crystals within the solubility limit of Cr which turned out to be also about 1%.",1505.05631v1 2016-11-22,Statistical Methods for Thermal Index Estimation Based on Accelerated Destructive Degradation Test Data,"Accelerated destructive degradation test (ADDT) is a technique that is commonly used by industries to access material's long-term properties. In many applications, the accelerating variable is usually the temperature. In such cases, a thermal index (TI) is used to indicate the strength of the material. For example, a TI of 200C may be interpreted as the material can be expected to maintain a specific property at a temperature of 200C for 100,000 hours. A material with a higher TI possesses a stronger resistance to thermal damage. In literature, there are three methods available to estimate the TI based on ADDT data, which are the traditional method based on the least-squares approach, the parametric method, and the semiparametric method. In this chapter, we provide a comprehensive review of the three methods and illustrate how the TI can be estimated based on different models. We also conduct comprehensive simulation studies to show the properties of different methods. We provide thorough discussions on the pros and cons of each method. The comparisons and discussion in this chapter can be useful for practitioners and future industrial standards.",1611.07412v1 2017-11-07,Fracture toughness characterization through notched small punch test specimens,"In this work a novel methodology for fracture toughness characterization by means of the small punch test (SPT) is presented. Notched specimens are employed and fracture resistance is assessed through a critical value of the notch mouth displacement {\delta^SPT}. Finite element simulations and interrupted experiments are used to track the evolution of {\delta^SPT} as a function of the punch displacement. The onset of crack propagation is identified by means of a ductile damage model and the outcome is compared to the crack tip opening displacement estimated from conventional tests at crack initiation. The proposed numerical-experimental scheme is examined with two different grades of CrMoV steel and the differences in material toughness captured. Limitations and uncertainties arising from the different damage phenomena observed in the lowest toughness material examined are thoroughly discussed.",1711.02406v1 2018-04-03,Combination of thermal and electric properties measurement techniques in a single setup suitable for radioactive materials in controlled environments and based on the 3-omega approach,"We have designed and developed a new experimental setup, based on the 3-omega method, to measure thermal conductivity, heat capacity and electrical resistivity of a variety of samples in a broad temperature range (2-550 K) and under magnetic fields up to 9 T. The validity of this method is tested by measuring various types of metallic (copper, platinum, and constantan) and insulating (SiO_2) materials, which have a wide range of thermal conductivity values (1-400 Wm-1K-1). We have successfully employed this technique for measuring the thermal conductivity of two actinide single crystals, uranium dioxide, and uranium nitride. This new experimental approach for studying nuclear materials will help to advance reactor fuel development and understanding. We have also shown that this experimental setup can be adapted to the Physical Property Measurement System (Quantum Design) environment and/or other cryocooler systems.",1804.00821v1 2018-11-02,Non-Equilibrium Phonon Transport Across Nanoscale Interfaces,"Despite the ubiquity of applications of heat transport across nanoscale interfaces, including integrated circuits, thermoelectrics, and nanotheranostics, an accurate description of phonon transport in these systems remains elusive. Here we present a theoretical and computational framework to describe phonon transport with position, momentum and scattering event resolution. We apply this framework to a single material spherical nanoparticle for which the multidimensional resolution offers insight into the physical origin of phonon thermalization, and length-scale dependent anisotropy of steady-state phonon distributions. We extend the formalism to handle interfaces explicitly and investigate the specific case of semi-coherent materials interfaces by computing the coupling between phonons and interfacial strain resulting from aperiodic array of misfit dislocations. Our framework quantitatively describes the thermal interface resistance within the technologically relevant Si-Ge heterostructures. In future, this formalism could provide new insight into coherent and driven phonon effects in nanoscale materials increasingly accessible via ultrafast, THz and near-field spectroscopies.",1811.01059v1 2018-11-07,Spin Hall effect in 2D metallic delafossite PtCoO$_2$ and vicinity topology,"The two-dimensional (2D) metal PtCoO$_2$ is renowned for the lowest room temperature resistivity among all oxides, close to that of the top two materials Ag and Cu. In addition, we theoretically predict a strong intrinsic spin Hall effect. This originates from six strongly-tilted Dirac cones that we find in the electronic structure near the Fermi surface, where a gap is opened by large spin-orbit coupling (SOC). This is underpinned by rich topological properties; in particular, the phenomenology of a mirror Chern metal is realized not exactly, but very accurately, on account of an approximate crystalline symmetry. We expect that such 'vicinity topology' to be a feature of relevance well beyond this material. Our Wilson loop analysis indicates further elaborate features such as fragile topology. These findings highlight PtCoO$_2$ as a promising material for spintronic applications as well as a platform to study the interplay of symmetry and topology.",1811.03105v1 2020-03-22,Thermoelectric probe of defect state induced by ionic liquid gating in vanadium dioxide,"Thermoelectric measurements detect the asymmetry between the density of states above and below the chemical potential in a material. It provides insights into small variations in the density of states near the chemical potential, complementing electron transport measurements. Here, combined resistance and thermoelectric power measurements are performed on vanadium dioxide (VO2), a prototypical correlated electron material, under ionic-liquid (IL) gating. With IL gating, charge transport below the metal-to-insulator-transition (MIT) temperature remains in the thermally activated regime, while the Seebeck coefficient exhibits an apparent transition from semiconducting to metallic behavior. The contrasting behavior indicates changes in electronic structure upon IL gating, due to the formation of oxygen defect states. The experimental results are corroborated by numerical simulations based on a model density of states incorporating a gating induced defect band. This study reveals thermoelectric measurements to be a convenient and sensitive probe for the role of defect states induced by IL gating in suppressing the MIT in VO2, which remains benign in charge transport measurements, and possibly for studying defect sates in other materials.",2003.09840v1 2017-03-10,Highly crystalline 2D superconductors,"Recent technological advances in controlling materials have developed methods to produce idealized two-dimensional (2D) electron systems such as heterogeneous interfaces, molecular-beam-epitaxy (MBE) grown atomic layers, exfoliated thin flakes and field-effect devices. These 2D electron systems are highly-crystalline with less disorder in common, some of which indeed show sheet resistance more than one order of magnitude lower even in atomic layers or single layers than that of conventional amorphous/granular thin films. Here, we present a review on the recent developments of highly-crystalline 2D superconductors and a series of unprecedented physical properties discovered in these systems. In particular, we highlight the quantum metallic state (or possible metallic ground state), the quantum Griffiths phase in out-of-plane magnetic fields, and the superconducting state maintained in anomalously large in-plane magnetic fields, which were observed in exfoliated 2D materials, MBE-grown atomic-layer thin films and electric-double-layer (ion-gated) interfaces. These phenomena are discussed on the basis of weakened disorder and/or broken spatial inversion symmetry. These novel aspects suggest that highly-crystalline 2D systems are promising platforms for exploring new quantum physics and superconductors.",1703.03541v1 2018-10-07,Log-periodic quantum magneto-oscillations and discrete scale invariance in topological material HfTe5,"Discrete scale invariance (DSI) is a phenomenon featuring intriguing log-periodicity which can be rarely observed in quantum systems. Here we report the log-periodic quantum oscillations in the magnetoresistance (MR) and the Hall traces of HfTe5 crystals, which reveals the appearance of DSI. The oscillations show the same logB-periodicity in the behavior of MR and Hall, indicating an overall effect of the DSI on the transport properties. Moreover, the DSI feature in the Hall resistance signals its close relation to the carriers. Combined with theoretical simulations, we further clarify the origin of the log-periodic oscillations and the DSI in the topological materials. Our work evidences the universality of the DSI in the Dirac materials and paves way for the full understanding of the novel phenomenon.",1810.03109v1 2019-02-20,Structural origins of electronic conduction in amorphous copper-doped alumina,"We perform an {\it ab initio} modeling of amorphous copper-doped alumina (a-Al$_2$O$_3$:Cu), a prospective memory material based on resistance switching, and study the structural origin of electronic conduction in this material. We generate molecular dynamics based models of a-Al$_2$O$_3$:Cu at various Cu-concentrations and study the structural, electronic and vibrational properties as a function of Cu-concentration. Cu atoms show a strong tendency to cluster in the alumina host, and metallize the system by filling the band gap uniformly for higher Cu-concentrations. We also study thermal fluctuations of the HOMO-LUMO energy splitting and observe the time evolution of the size of the band gap, which can be expected to have an important impact on the conductivity. We perform a numerical computation of conduction pathways, and show its explicit dependence on Cu connectivity in the host. We present an analysis of ion dynamics and structural aspects of localization of classical normal modes in our models.",1902.07559v1 2017-04-03,Superconducting Two-Dimensional Metal-Organic Framework,"Superconductivity is a fascinating quantum phenomenon characterized by zero electrical resistance and the Meissner effect. To date, several distinct families of superconductors (SCs) have been discovered. These include three-dimensional (3D) bulk SCs in both inorganic and organic materials as well as two-dimensional (2D) thin film SCs but only in $inorganic$ materials. Here we predict superconductivity in 2D and 3D $organic$ metal-organic frameworks by using first-principles calculations. We show that the highly conductive and recently synthesized Cu-benzenehexathial (BHT) is a Bardeen-Cooper-Schrieffer SC. Remarkably, the monolayer Cu-BHT has a critical temperature ($T_{c}$) of 4.43 K while $T_{c}$ of bulk Cu-BHT is 1.58 K. Different from the enhanced $T_{c}$ in 2D inorganic SCs which is induced by interfacial effects, the $T_{c}$ enhancement in this 2D organic SC is revealed to be the out-of-plane soft-mode vibrations, analogous to surface mode enhancement originally proposed by $Ginzburg$. Our findings not only shed new light on better understanding 2D superconductivity, but also open a new direction to search for SCs by interface engineering with organic materials.",1704.00490v1 2019-08-07,Transport phenomena in a free-standing two-dimensional sodium sheet,"The advances in the growth techniques provide numerous scope to explore the possibilities of new 2D materials for potential applications. With the aid of first-principle calculations we show that 2D Na can be a new addition to the family of thermodynamically stable 2D materials for device applications. Not surprisingly, due to half-occupied $3s$ orbital 2D Na possesses the features of the 2D electron gas (2DEG). The transport properties are examined based on the accurate solution of Boltzmann transport equation. With practically tunable carrier density in 2D materials, the intrinsic electrical resistivity of electron doped 2D Na is $\sim$ 1.4 times larger than that of graphene and falls below the latter 450 K onwards. The Bloch-Gr\""uneisen temperature is almost constant at 50 K, independent of the type or density of the charge carriers. The electronic thermal conductivity of pure 2D Na is $\sim$ 1.24 times larger than that of its bulk counterpart at 300 K. The Wiedemann-Franz law stands tall in 2D Na with calculated Lorenz number 2.41 $\times 10^{-8} V^2/deg^2$ at room temperature. The transport mechanism presented here is expected to occur in all Na like systems with a clean Fermi surface.",1908.02431v1 2019-12-18,Observation of multiple Dirac states in a magnetic topological material EuMg2Bi2,"Initiated by the discovery of topological insulators, topologically non-trivial materials, more specifically topological semimetals and metals have emerged as new frontiers in the field of quantum materials. In this work, we perform a systematic measurement of EuMg2Bi2, a compound with antiferromagnetic transition temperature at 6.7 K, observed via electrical resistivity, magnetization and specific heat capacity measurements. By utilizing angle-resolved photoemission spectroscopy in concurrence with first-principles calculations, we observe Dirac cones at the corner and the zone center of the Brillouin zone. From our experimental data, multiple Dirac states at G and K points are observed, where the Dirac nodes are located at different energy positions from the Fermi level. Our experimental investigations of detailed electronic structure as well as transport measurements of EuMg2Bi2 suggest that it could potentially provide a platform to study the interplay between topology and magnetism.",1912.08645v1 2012-03-28,Finite element modelling of shock-induced damages on ceramic hip prostheses,"The aim of this work was to simulate the behaviour of hip prostheses under mechanical shocks. When hip joint is replaced by prosthesis, during the swing phase of the leg, a microseparation between the prosthetic head and the cup could occur. Two different sizes of femoral heads were studied: 28 and 32 mm diameter, made, respectively, in alumina and zirconia. The shock-induced stress was determined numerically using finite element analysis (FEA), Abaqus software. The influence of inclination, force, material, and microseparation was studied. In addition, an algorithm was developed from a probabilistic model, Todinov's approach, to predict lifetime of head and cup. Simulations showed maximum tensile stresses were reached on the cup's surfaces near to rim. The worst case was the cup-head mounted at 30^{\circ}. All simulations and tests showed bulk zirconia had a greater resistance to shocks than bulk alumina. The probability of failure could be bigger than 0.9 when a porosity greater than 0.7% vol. is present in the material. Simulating results showed good agreement with experimental results. The tests and simulations are promising for predicting the lifetime of ceramic prostheses.",1203.6154v1 2015-04-20,Giant reversible nanoscale piezoresistance at room temperature in Sr2IrO4 thin films,"Layered iridates have been the subject of intense scrutiny on account of their unusually strong spin-orbit coupling, which opens up a narrow gap in a material that would otherwise be a metal. This insulating state is very sensitive to external perturbations. Here, we show that vertical compression at the nanoscale, delivered using the tip of a standard scanning probe microscope, is capable of inducing a five orders of magnitude change in the room temperature resistivity of Sr2IrO4. The extreme sensitivity of the electronic structure to anisotropic deformations opens up a new angle of interest on this material, and the giant and fully reversible perpendicular piezoresistance makes iridates a promising material for room temperature piezotronic devices.",1504.05245v1 2018-12-06,Crack Growth Behavior in NiTi Shape Memory Alloys Under Mode-I Isothermal Loading: Effect of Stress State,"Fracture behavior in nickel-titanium (NiTi) shape memory alloys (SMAs) subjected to mode-I, isothermal loading is studied using finite element analysis (FEA). Compact tension (CT) SMA specimen is modeled in Abaqus finite element suite and crack growth under displacement boundary condition is investigated for plane strain and plane stress conditions. Parameters for the SMA material constitutive law implemented in the finite element setup are acquired from characterization tests conducted on near-equiatomic NiTi SMA. Virtual crack closure technique (VCCT) is implemented where crack is assumed to extend when the energy release rate at the crack-tip becomes equal to the experimentally obtained material-specific critical value. Load-displacement curves and mechanical fields near the crack-tip in plane strain and plane stress cases are examined. Moreover, a discussion with respect to the crack resistance R-curves calculated using the load-displacement response for plane strain and plane stress conditions is presented.",1812.02362v1 2018-12-24,Control of Spin Diffusion and Suppression of the Hanle Effect by the Coexistence of Spin and Valley Hall Effects,"In addition to spin, electrons in many materials possess an additional pseudo-spin degree of freedom known as 'valley'. In materials where the spin and valley degrees of freedom are weakly coupled, they can be both excited and controlled independently. In this work, we study a model describing the interplay of the spin and valley Hall effects in such two-dimensional materials. We demonstrate the emergence of an additional longitudinal neutral current that is both spin and valley polarized. The additional neutral current allows to control the spin density by tuning the magnitude of the valley Hall effect. In addition, the interplay of the two effects can suppress the Hanle effect, that is, the oscillation of the nonlocal resistance of a Hall bar device with in-plane magnetic field. The latter observation provides a possible explanation for the absence of the Hanle effect in a number of recent experiments. Our work opens also the possibility to engineer the conversion between the valley and spin degrees of freedom in two-dimensional materials.",1812.09996v2 2019-06-24,Cross interface model for the thermal transport across interface between overlapped boron nitride nanoribbons,"The application of low-dimensional materials for heat dissipation requires a comprehensive understanding of the thermal transport at the cross interface, which widely exists in various composite materials and electronic devices. In this work, we proposed an analytical model, named as cross interface model (CIM), to accurately reveal the essential mechanism of the two-dimensional thermal transport at the cross interface. The applicability of CIM is validated through the comparison of the analytical results with molecular dynamics simulations for a typical cross interface of two overlapped boron nitride nanoribbons. Besides, it is figured out that the factor ({\eta}) has important influence on the thermal transport besides the thermal resistance inside and between the materials, which is found to be determined by two dimensionless parameters from its expression. Our investigations deepen the understanding of the thermal transport at the cross interface and also facilitate to guide the applications of low-dimensional materials in thermal management.",1906.09751v1 2019-11-05,Molecular beam epitaxy of CuMnAs,"We present a detailed study of the growth of the tetragonal polymorph of antiferromagnetic CuMnAs by the molecular beam epitaxy technique. We explore the parameter space of growth conditions and their effect on the microstructural and transport properties of the material. We identify its typical structural defects and compare the properties of epitaxial CuMnAs layers grown on GaP, GaAs and Si substrates. Finally, we investigate the correlation between the crystalline quality of CuMnAs and its performance in terms of electrically induced resistance switching.",1911.01794v1 2019-11-15,Flexoskeleton printing for versatile insect-inspired robots,"One of the many secrets to the success and prevalence of insects is their versatile, robust, and complex exoskeleton morphology. A fundamental challenge in insect-inspired robotics has been the fabrication of robotic exoskeletons that can match the complexity of exoskeleton structural mechanics. Hybrid robots composed of rigid and soft elements have previously required access to expensive multi-material 3D printers, multi-step casting and machining processes, or limited material choice when using consumer-grade fabrication methods. Here we introduce a new design and fabrication process to rapidly construct flexible exoskeleton-inspired robots called flexoskeleton printing. We modify a consumer-grade fused deposition material (FDM) 3D printer to deposit filament directly onto a heated thermoplastic base layer which provides extremely strong bond strength between the deposited material and the inextensible, flexible base layer. This process significantly improves the fatigue resistance of printed components and enables a new class of insect-inspired robot morphologies. We demonstrate these capabilities through design and testing of a wide library of canonical flexoskeleton elements; ultimately leading to the integration of elements into a flexoskeleton walking legged robot.",1911.06897v2 2020-01-07,Molecular beam epitaxy of the magnetic kagome metal FeSn on LaAlO3 (111),"Materials with a layered Kagome lattice are expected to give rise to novel physics arising from band structures with topological properties, spin liquid behavior and the formation of skyrmions. Until now, most work on Kagome materials has been performed on bulk samples due to difficulties in thin film synthesis. Here, by using molecular beam epitaxy, layered Kagome-structured FeSn films are synthesized on (111) oriented LaAlO3 substrate. Both in-situ and ex-situ characterizations indicate these films are highly crystalline and c-axis oriented, with atomically smooth surfaces. However, the films grow as disconnected islands, with lateral dimensions on the micron scale. By patterning Pt electrodes using a focused electron beam, longitudinal and transverse resistance of single islands have been measured in magnetic fields. Our work opens a pathway for exploring mesoscale transport properties in thin films of Kagome materials and related devices.",2001.01820v2 2020-05-11,Highly flexible electromagnetic interference shielding films based on ultrathin Ni/Ag composites on paper substrates,"Highly flexible electromagnetic interference (EMI) shielding material with excellent shielding performance is of great significance to practical applications in next-generation flexible devices. However, most EMI materials suffer from insufficient flexibility and complicated preparation methods. In this study, we propose a new scheme to fabricate a magnetic Ni particle/Ag matrix composite ultrathin film on a paper surface. For a ~2 micro meter thick film on paper, the EMI shielding effectiveness (SE) was found to be 46.2 dB at 8.1 GHz after bending 200,000 times over a radius of ~2 mm. The sheet resistance (Rsq) remained lower than 2.30 Ohm after bending 200,000 times. Contrary to the change in Rsq, the EMI SE of the film generally increased as the weight ratio of Ag to Ni increased, in accordance with the principle that EMI SE is positively related with an increase in electrical conductivity. Desirable EMI shielding ability, ultrahigh flexibility, and simple processing provide this material with excellent application prospects.",2005.04875v1 2020-08-19,Observation of plateau-like magnetoresistance in twisted Fe3GeTe2/Fe3GeTe2 junction,"Controlling the stacking of van der Waals (vdW) materials is found to produce exciting new findings, since hetero- or homo- structures have added the diverse possibility of assembly and manipulated functionalities. However, so far, the homostructure with a twisted angle based on the magnetic vdW materials remains unexplored. Here, we achieved a twisted magnetic vdW Fe3GeTe2/Fe3GeTe2 junction with broken crystalline symmetry. A clean and metallic vdW junction is evidenced by the temperature-dependent resistance and the linear I-V curve. Unlike the pristine FGT, a plateau-like magnetoresistance (PMR) is observed in the magnetotransport of our homojunction due to the antiparallel magnetic configurations of the two FGT layers. The PMR ratio is found to be ~0.05% and gets monotonically enhanced as temperature decreases like a metallic giant magnetoresistance (GMR). Such a tiny PMR ratio is at least three orders of magnitude smaller than the tunneling magnetoresistance (TMR) ratio, justifying our clean metallic junction without a spacer. Our findings demonstrate the feasibility of the controllable homostructure and shed light on future spintronics using magnetic vdW materials.",2008.08313v1 2020-10-24,Drawing WS2 thermal sensors on paper substrates,"Paper based thermoresistive sensors are fabricated by rubbing WS2 powder against a piece of standard copier paper, like the way a pencil is used to write on paper. The abrasion between the layered material and the rough paper surface erodes the material, breaking the weak van der Waals interlayer bonds, yielding a film of interconnected platelets. The resistance of WS2 presents a strong temperature dependence, as expected for a semiconductor material in which charge transport is due to thermally activated carriers. This strong temperature dependence makes the paper supported WS2 devices extremely sensitive to small changes in temperature. This exquisite thermal sensitivity, and their fast response times to sudden temperature changes, is exploited thereby demonstrating the usability of a WS2-on-paper thermal sensor in a respiration monitoring device.",2010.12805v1 2021-04-08,Correlating Nanocrystalline Structure with Electronic Properties in 2D Platinum Diselenide,"Platinum diselenide (PtSe${_2}$) is a two-dimensional (2D) material with outstanding electronic and piezoresistive properties. The material can be grown at low temperatures in a scalable manner which makes it extremely appealing for many potential electronics, photonics, and sensing applications. Here, we investigate the nanocrystalline structure of different PtSe${_2}$ thin films grown by thermally assisted conversion (TAC) and correlate them with their electronic and piezoresistive properties. We use scanning transmission electron microscopy for structural analysis, X-ray photoelectron spectroscopy (XPS) for chemical analysis, and Raman spectroscopy for phase identification. Electronic devices are fabricated using transferred PtSe${_2}$ films for electrical characterization and piezoresistive gauge factor measurements. The variations of crystallite size and their orientations are found to have a strong correlation with the electronic and piezoresistive properties of the films, especially the sheet resistivity and the effective charge carrier mobility. Our findings may pave the way for tuning and optimizing the properties of TAC-grown PtSe${_2}$ towards numerous applications.",2104.03636v1 2021-09-16,Analytic solution to pseudo-Landau levels in strongly bent graphene nanoribbons,"Nonuniform elastic strain is known to induce pseudo-Landau levels in Dirac materials. But these pseudo-Landau levels are hardly resolvable in an analytic fashion when the strain is strong, because of the emerging complicated space dependence in both the strain-modulated Fermi velocity and the strain-induced pseudomagnetic field. We analytically characterize the solution to the pseudo-Landau levels in experimentally accessible strongly bent graphene nanoribbons, by treating the effects of the nonuniform Fermi velocity and pseudomagnetic field on equal footing. The analytic solution is detectable through the angle-resolved photoemission spectroscopy (ARPES) and allows quantitative comparison between theories and various transport experiments, such as the Shubnikov-de Haas oscillation in the complete absence of magnetic fields and the negative strain-resistivity resulting from the valley anomaly. The analytic solution can be generalized to twisted two-dimensional materials and topological materials and will shed a new light on the related experimental explorations and straintronics applications.",2109.08182v2 2021-09-27,"Layered, Tunable Graphene Oxide-Nylon Heterostructures for Wearable Electrocardiogram Sensors","Nanoscale engineered materials combined with wearable wireless technologies can deliver a new level of health monitoring. A reduced graphene oxide-nylon composite material is developed and tested, demonstrating its usefulness as a material for sensors in wearable, long-term electrocardiogram (ECG) monitoring via a comparison to one of the widely used ECG sensors. The structural analysis by scanning electron (SEM) and atomic force microscopy (AFM) shows a limited number of defects on a macroscopic scale. Fourier Transform Infrared (FTIR) and Raman spectroscopy confirm the presence of rGOx, and the ratio of D- and G-features as a function of thickness correlates with the resistivity analysis. The negligible effect of the defects and the tunability of electrical and optical properties, together with live ECG data, demonstrate its signal transduction capability.",2109.12739v2 2022-04-30,Scattering mechanisms in state-of-the-art GaAs/AlGaAs quantum wells,"Motivated by recent breakthrough in molecular beam epitaxy of GaAs/AlGaAs quantum wells [Y. J. Chung \textit{et al.}, Nature Materials \textbf{20}, 632 (2021)], we examine contributions to mobility and quantum mobility from various scattering mechanisms and their dependencies on the electron density. We find that at lower electron densities, $n_e \lesssim 1 \times 10^{11}$ cm$^{-2}$, both transport and quantum mobility are limited by unintentional background impurities and follow a power law dependence, $\propto n_e^{\alpha}$, with $\alpha \approx 0.85$. Our predictions for quantum mobility are in reasonable agreement with an estimate obtained from the resistivity at filling factor $\nu= 1/2$ in a sample of Y. J. Chung \textit{et al.} with $n_e = 1 \times 10^{11}$ cm$^{-2}$. Consideration of other scattering mechanisms indicates that interface roughness (remote donors) is a likely limiting factor of transport (quantum) mobility at higher electron densities. Future measurements of quantum mobility should yield information on the distribution of background impurities in GaAs and AlGaAs.",2205.00365v3 2023-07-20,Superconductivity in a van der Waals layered quasicrystal,"van der Waals (vdW) layered transition-metal chalcogenides are attracting significant attention owing to their fascinating physical properties. This group of materials consists of abundant members with various elements, having a variety of different structures. However, all vdW layered materials studied to date have been limited to crystalline materials, and the physical properties of vdW layered quasicrystals have not yet been reported. Here, we report on the discovery of superconductivity in a vdW layered quasicrystal of Ta1.6Te. The electrical resistivity, magnetic susceptibility, and specific heat of the Ta1.6Te quasicrystal fabricated by reaction sintering, unambiguously validated the occurrence of bulk superconductivity at a transition temperature of ~1 K. This discovery can pioneer new research on assessing the physical properties of vdW layered quasicrystals as well as two-dimensional quasicrystals; moreover, it paves the way toward new frontiers of superconductivity in thermodynamically stable quasicrystals, which has been the predominant challenge facing condensed matter physics since the discovery of quasicrystals almost four decades ago.",2307.10679v1 2023-08-21,Coupling Between Magnetic and Transport Properties in Magnetic Layered Material Mn2-xZnxSb,"We synthesized single crystals for Mn2-xZnxSb and studied their magnetic and electronic transport properties. This material system displays rich magnetic phase tunable with temperature and Zn composition. In addition, two groups of distinct magnetic and electronic properties, separated by a critical Zn composition of x = 0.6, are discovered. The Zn-less samples are metallic and characterized by a resistivity jump at the magnetic ordering temperature, while the Zn-rich samples lose metallicity and show a metal-to-insulator transition-like feature tunable by magnetic field. Our findings establish Mn2-xZnxSb as a promising material platform that offers opportunities to study how the coupling of spin, charge, and lattice degrees of freedom governs interesting transport properties in 2D magnets, which is currently a topic of broad interest.",2308.10764v1 2023-10-08,An innovative clay metaBrick-based motif to enhance thermal and acoustic insulation,"Metamaterials have gained popularity in recent years as a promising avenue for producing innovative materials with distinctive properties that offer unprecedented features. In this study, we address the thermal and acoustic challenges of building materials. We numerically and experimentally investigate a clay metaBrick, which is an innovative metamaterial design based on the existing hollow brick that has shown strong sound and thermal performances. We evaluate the acoustic and thermal characteristics of the clay metaBrick, including sound transmission and heat resistance, using the finite element method. Furthermore, we validate the results experimentally by investigating the behaviors of the wall built on metaBricks in two tests: sound and thermal. We contrast the findings of the metaBrick based wall with performances of a standard hollow brick wall. The metaBrick offers enhanced acoustic and thermal insulation properties compared to the standard brick, with a compressive strength above standards required in the building materials.",2310.05148v1 2024-03-18,The Role of Temperature on Irradiation Defect Evolution near Surfaces and Grain Boundaries in Tungsten,"This study explores the impact of temperature on defect dynamics in tungsten, emphasizing its application in nuclear fusion reactors as Plasma Facing Components (PFCs). Through atomistic simulations, the research elucidates the intricate interplay of defect production, annihilation, and redistribution under irradiation at room (300K) and elevated temperatures (1000K). It demonstrates that higher temperatures significantly increase the number and mobility of defects, leading to a substantial rise in the total number of surviving Frenkel Pairs (FPs), with a notable preference for surface distribution. This redistribution is attributed to energy gradient-driven relocation processes, enhanced by the defects' increased mobility at elevated temperatures. Moreover, the study reveals that elevated temperatures promote biased accumulation of interstitial defects in grain boundaries, especially in configurations that facilitate efficient interstitial migration, indicating a strategy for minimizing lattice interstitial accumulation under irradiation. These findings underscore the critical role of temperature in modulating irradiation-induced defect dynamics in tungsten, providing valuable insights for designing and selecting materials with optimized irradiation resistance for use in extreme conditions of nuclear fusion reactors. The research suggests a material design approach that accounts for temperature effects to enhance the durability and performance of nuclear fusion materials.",2403.12259v1 2024-03-19,Unveiling the Reactivity of Oxygen and Ozone on C2N Monolayer: A First-Principles Study,"The process of environmental oxidation is pivotal in determining the physical and chemical properties of two-dimensional (2D) materials. Its impact holds great significance for the practical application of these materials in nanoscale devices functioning under ambient conditions. This study delves into the influence of O2 and O3 exposure on the structural and electronic characteristics of the C2N monolayer, focusing on the kinetics of adsorption and dissociation reactions. Employing first-principles density functional theory calculations alongside climbing image nudged elastic band calculations, we observe that the C2N monolayer exhibits resistance to oxidation and ozonation, evidenced by energy barriers of 0.05 eV and 0.56 eV, respectively. These processes are accompanied by the formation of epoxide (C-O-C) groups. Furthermore, the dissociation mechanism involves charge transfers from the monolayer to the molecules. Notably, the dissociated configurations demonstrate higher bandgaps compared to the pristine C2N monolayer, attributed to robust C-O hybridization. These findings suggest the robustness of C2N monolayers against oxygen/ozone exposures, ensuring stability for devices incorporating these materials.",2403.12454v1 2024-05-13,Significant improvement in sensitivity of an anomalous Nernst heat flux sensor by composite structure,"Heat flux sensors (HFS) have attracted significant interest for their potential in managing waste heat efficiently. A recently proposed HFS, that works on the basis of the anomalous Nernst effect (ANE), offers several advantages in its simple structure leading to easy fabrication, low cost, and reduced thermal resistance. However, enhancing sensitivity through traditional material selection is now challenging due to a small number of materials satisfying the required coexistence of a large transverse Seebeck coefficient and low thermal conductivity. In this study, by utilizing composite structures and optimizing the device geometry, we have achieved a substantial improvement in the sensitivity of an ANE-based HFS. We developed composite structures comprised of a plastic substrate with an uneven surface and three-dimensional (3D) uneven TbCo films, fabricated using nanoimprint techniques and sputtering. This approach resulted in a sensitivity that is approximately four times greater than that observed in previous studies. Importantly, this method is independent of the material properties and can significantly enhance the sensitivity. Our findings could lead to the development of highly sensitive HFS devices and open new avenues for the fabrication of 3D devices.",2405.07758v1 2003-08-25,Formation of Semi-relativisitc Jets from Magnetospheres of Accreting Neutron Stars: Injection of Hot Bubbles into a Magnetic Tower,"We present the results of 2.5-dimensional resistive magnetohydrodynamic (MHD) simulations of the magnetic interaction between a weakly magnetized neutron star and its accretion disk. General relativistic effects are simulated by using the pseudo-Newtonian potential. We find that well-collimated jets traveling along the rotation axis of the disk are formed by the following mechanism: (1) The magnetic loops connecting the neutron star and the disk are twisted due to the differential rotation between the neutron star and the disk. (2) Twist injection from the disk initiates expansion of the loop. (3) The expanding magnetic loops create a magnetic tower in which accelerated disk material travel as collimated bipolar jets. The propagation speed of the working surface of the jet is the order of 10% of the speed of light ($\sim 0.1c$). (4) Magnetic reconnection taking place inside the expanding magnetic loops injects hot bubbles intermittently into the magnetic tower. The ejection speed of the bubble is the order of the local Alfv\'{e}n speed of the launching point and $\sim 0.2c$ in our simulations. (5) The hot bubbles moving inside the tower catch up with the working surface of the jet. High energy electrons created by the magnetic reconnection are a plausible source of radio emission. Our model can explain the formation process of a narrow jet from a weakly magnetized ($|{\boldmath$B_{*}$}|\le 10^{9}$ gauss) neutron star and the correlation between radio flares of the core and of the lobe observed in Sco X-1.",0308437v2 2009-01-28,Strong enhancement of Jc in binary and alloyed in-situ MgB2 wires by a new approach: Cold high pressure densification,"Cold high pressure densification (CHPD) is presented as a new way to substantially enhance the critical current density of in situ MgB2 wires at 4.2 and 20 K at fields between 5 and 14 T. The results on two binary MgB2 wires and an alloyed wire with 10 wt.% B4C are presented The strongest enhancement was measured at 20K, where cold densification at 1.85 GPa on a binary Fe/MgB2 wire raised both Jcpara and Jcperp by more than 300% at 5T, while Birr was enhanced by 0.7 T. At 4.2K, the enhancement of Jc was smaller, but still reached 53% at 10 T. After applying pressures up to 6.5 GPa, the mass density dm of the unreacted (B+Mg) mixture inside the filaments reached 96% of the theoretical density. After reaction under atmospheric pressure, this corresponds to a highest mass density df in the MgB2 filaments of 73%. After reaction, the electrical resistance of wires submitted to cold densification was found to decrease, reflecting an improved connectivity. A quantitative correlation between filament mass density and the physical properties was established. Monofilamentary rectangular wires with aspect ratios a/b < 1.25 based on low energy ball milled powders exhibited very low anisotropy ratios, Gamma = Jcpara/Jcperp being < 1.4 at 4.2 K and 10T. The present results can be generalized to alloyed MgB2 wires, as demonstrated on a wire with B4C additives. Based on the present data, it follows that cold densification has the potential of further improving the highest Jcpara and Jcperp values reported so far for in situ MgB2 tapes and wires with SiC and C additives. Investigations are under work in our laboratory to determine whether the densification method CHPD can be applied to longer wire or tape lengths.",0901.4546v1 2011-01-24,"Stabilization of an ambient pressure, collapsed tetragonal phase in CaFe2As2 and tuning of the orthorhombic / antiferromagnetic transition temperature by over 70 K by control of nano-precipitates","We have found a remarkably large response of the transition temperature of CaFe2As2 single crystals grown out of excess FeAs to annealing / quenching temperature. Whereas crystals that are annealed at 400 C exhibit a first order phase transition from a high temperature tetragonal to a low temperature orthorhombic and antiferromagnetic state near 170 K, crystals that have been quenched from 960 C exhibit a transition from a high temperature tetragonal phase to a low temperature, non-magnetic, collapsed tetragonal phase below 100 K. By use of temperature dependent electrical resistivity, magnetic susceptibility, X-ray diffraction, Mossbauer spectroscopy and nuclear magnetic resonance measurements we have been able to demonstrate that the transition temperature can be reduced in a monotonic fashion by varying the annealing / quenching temperature from 400 to 850 C with the low temperature state remaining antiferromagnetic for transition temperatures larger than 100 K and becoming collapsed tetragonal / non-magnetic for transition temperatures below 90 K. This suppression of the orthorhombic / antiferromagnetic phase transition and its ultimate replacement with the collapsed tetragonal / non-magnetic phase is similar to what has been observed for CaFe2As2 under hydrostatic pressure. Transmission electron microscopy studies indicate that there is a temperature dependent, width of formation of CaFe2As2 with a decreasing amount of excess Fe and As being soluble in the single crystal at lower annealing temperatures. For samples quenched from 960 C there is a fine (of order 10 nm), semi-uniform distribution of precipitate that can be associated with an average strain field whereas for samples annealed at 400 C the excess Fe and As form mesoscopic grains that induce little strain throughout the CaFe2As2 lattice.",1101.4595v1 2011-10-14,Numerical Investigation of Design Strategies to Achieve Long-Life Pavements,"Increasing the HMA base thickness and modifying the HMA mixture properties to improve the resistance to fatigue cracking are among the most popular methods for achieving long-lasting pavements. Such methods are based on the idea of reducing the tensile strain at the bottom of the HMA layer below the Fatigue Endurance Limit (FEL), a level of strain below which no cumulative damage occurs to the HMA mixture. This study investigates the effectiveness of several design strategies involved in long-life, perpetual pavement design. A 3D Finite Element model of the pavement involving a linear viscoelastic constitutive model for HMA materials and non-uniform tire contact stresses is developed using ABAQUS 6.11. The effects of asphalt base course thickness and mixture type, rich binder layer, and aggregate subbase layer are examined. Four asphalt base course mixture types, namely dense graded, polymer modified, high modulus, and standard binder, are studied as a function of the asphalt base course thickness. The results underline a better performance of the high-modulus asphalt base, as compared to the other base course mixtures. The aggregate subbase layer on top of subgrade soil showed a relatively minor effect on the longitudinal and lateral strain response at the bottom of asphalt base course. The addition of a rich binder layer at the bottom of the asphalt base course showed a significant reduction in tensile strains. Tables are provided as a guideline to assess the different alternatives in design of long-life perpetual pavements.",1110.3318v7 2013-06-21,"Crystallographic, Electronic, Thermal and Magnetic Properties of Single-Crystal SrCo2As2","In tetragonal SrCo2As2 single crystals, inelastic neutron scattering measurements demonstrated that strong stripe-type antiferromagnetic (AFM) correlations occur at a temperature T = 5 K [W. Jayasekara et al., arXiv:1306.5174] that are the same as in the isostructural AFe2As2 (A = Ca, Sr, Ba) parent compounds of high-Tc superconductors. This surprising discovery suggests that SrCo2As2 may also be a good parent compound for high-Tc superconductivity. Here, structural and thermal expansion, electrical resistivity rho, angle-resolved photoemission spectroscopy (ARPES), heat capacity Cp, magnetic susceptibility chi, 75As NMR and neutron diffraction measurements of SrCo2As2 crystals are reported together with LDA band structure calculations that shed further light on this fascinating material. The c-axis thermal expansion coefficient alpha_c is negative from 7 to 300 K, whereas alpha_a is positive over this T range. The rho(T) shows metallic character. The ARPES measurements and band theory confirm the metallic character and in addition show the presence of a flat band near the Fermi energy E_F. The band calculations exhibit an extremely sharp peak in the density of states D(E_F) arising from a flat d_{x^2 - y^2} band. A comparison of the Sommerfeld coefficient of the electronic specific heat with chi(T = 0) suggests the presence of strong ferromagnetic itinerant spin correlations which on the basis of the Stoner criterion predicts that SrCo2As2 should be an itinerant ferromagnet, in conflict with the magnetization data. The chi(T) does have a large magnitude, but also exhibits a broad maximum at 115 K suggestive of dynamic short-range AFM spin correlations, in agreement with the neutron scattering data. The measurements show no evidence for any type of phase transition between 1.3 and 300 K and we propose that metallic SrCo2As2 has a gapless quantum spin-liquid ground state.",1306.5222v3 2014-02-17,Unravelling the effect of SrTiO3 antiferrodistortive phase transition on the magnetic properties of La0.7Sr0.3MnO3 thin films,"Epitaxial La0.7Sr0.3MnO3 (LSMO) thin films, with different thickness ranging from 20 nm up to 330 nm, were deposited on (100)-oriented strontium titanate (STO) substrates by pulsed laser deposition, and their structure and morphology characterized at room temperature. Magnetic and electric transport properties of the as-processed thin films reveal an abnormal behavior in the temperature dependent magnetization M(T) below the antiferrodistortive STO phase transition (TSTO) and also an anomaly in the magnetoresistance and electrical resistivity close to the same temperature. Up to 100 nm LSMO thin films, an in-excess magnetization and pronounced changes in the coercivity are evidenced, achieved through the interface-mediated magnetoelastic coupling with antiferrodistortive domain wall movement occurring below TSTO. Contrarily, for thicker LSMO thin films, above 100 nm, an in-defect magnetization is observed. This reversed behavior can be understood within the emergence in the upper layer of the film, observed by high resolution transmission electron microscopy, of a branched structure needed to relax elastic energy stored in the film which leads to randomly oriented magnetic domain reconstructions. For enough high-applied magnetic fields, as thermodynamic equilibrium is reached, a fully suppression of the anomalous magnetization occurs, wherein the temperature dependence of the magnetization starts to follow the expected Brillouin behavior.",1402.4040v1 2017-12-04,Effect of crystalline anisotropy on vertical (-201) and (010) beta-Ga2O3 Schottky barrier diodes on EFG single-crystal substrates,"Vertical (-201) and (010) beta-Ga2O3 Schottky barrier diodes (SBDs) were fabricated on single-crystal substrates grown by edge-defined film-fed growth (EFG) method. High resolution X-ray diffraction (HRXRD) and atomic force microscopy (AFM) confirmed good crystal quality and surface morphology of the substrates. The electrical properties of both devices, including current-voltage (I-V) and capacitance-voltage (C-V) characteristics, were comprehensively measured and compared. The (-201) and (010) SBDs exhibited on-resistances (Ron) of 0.56 and 0.77 m{\Omega}cm2, turn-on voltages (Von) of 1.0 and 1.3 V, Schottky barrier heights (SBH) of 1.05 and 1.20 eV, electron mobilities of 125 and 65 cm2/(Vs), respectively, with a high on-current of ~1.3 kA/cm2 and on/off ratio of ~109. The (010) SBD had a larger Von and SBH than (-201) SBD due to anisotropic surface properties (i.e., surface Fermi level pinning and band bending), as supported by X-ray photoelectron spectroscopy (XPS) measurements. Temperature-dependent I-V also revealed the inhomogeneous nature of the SBH in both devices, where (-201) SBD showed a more uniform SBH distribution. The homogeneous SBH was also extracted: 1.33 eV for (-201) SBD and 1.53 eV for (010) SBD. The reverse leakage current of the devices was well described by the two-step trap-assisted tunneling model and the one-dimensional variable range hopping conduction (1D-VRH) model. The (-201) SBD showed larger leakage current due to its lower SBH and smaller activation energy. These results indicate the crystalline anisotropy of beta-Ga2O3 can affect the electrical properties of vertical SBDs and should be taken into consideration when designing beta-Ga2O3 electronics.",1712.01318v1 2018-04-30,Detailed study on the Fermi surfaces of the type-II Dirac semimetallic candidates PdTe2 and PtTe2,"We present a detailed quantum oscillatory study on the Dirac type-II semimetallic candidates PdTe$_{2}$ and PtTe$_{2}$ \emph{via} the temperature and the angular dependence of the de Haas-van Alphen (dHvA) and Shubnikov-de Haas (SdH) effects. In high quality single crystals of both compounds, i.e. displaying carrier mobilities between $10^3$ and $10^4$ cm$^2$/Vs, we observed a large non-saturating magnetoresistivity (MR) which in PtTe$_2$ at a temperature $T = 1.3$ K, leads to an increase in the resistivity up to $5 \times 10^{4}$ % under a magnetic field $\mu_0 H = 62$ T. These high mobilities correlate with their light effective masses in the range of 0.04 to 1 bare electron mass according to our measurements. For PdTe$_{2}$ the experimentally determined Fermi surface cross-sectional areas show an excellent agreement with those resulting from band-structure calculations. Surprisingly, this is not the case for PtTe$_{2}$ whose agreement between calculations and experiments is relatively poor even when electronic correlations are included in the calculations. Therefore, our study provides a strong support for the existence of a Dirac type-II node in PdTe$_2$ and probably also for PtTe$_2$. Band structure calculations indicate that the topologically non-trivial bands of PtTe$_2$ do not cross the Fermi-level ($\varepsilon_F$). In contrast, for PdTe$_2$ the Dirac type-II cone does intersect $\varepsilon_F$, although our calculations also indicate that the associated cyclotron orbit on the Fermi surface is located in a distinct $k_z$ plane with respect to the one of the Dirac type-II node. Therefore it should yield a trivial Berry-phase.",1805.00087v1 2017-03-20,Pseudogap temperature $T^\star$ of cuprate superconductors from the Nernst effect,"We use the Nernst effect to delineate the boundary of the pseudogap phase in the temperature-doping phase diagram of cuprate superconductors. New data for the Nernst coefficient $\nu(T)$ of YBa$_{2}$Cu$_{3}$O$_{y}$ (YBCO), La$_{1.8-x}$Eu$_{0.2}$Sr$_x$CuO$_4$ (Eu-LSCO) and La$_{1.6-x}$Nd$_{0.4}$Sr$_x$CuO$_4$ (Nd-LSCO) are presented and compared with previous data including La$_{2-x}$Sr$_x$CuO$_4$ (LSCO). The temperature $T_\nu$ at which $\nu/T$ deviates from its high-temperature behaviour is found to coincide with the temperature at which the resistivity deviates from its linear-$T$ dependence, which we take as the definition of the pseudogap temperature $T^\star$- in agreement with gap opening detected in ARPES data. We track $T^\star$ as a function of doping and find that it decreases linearly vs $p$ in all four materials, having the same value in the three LSCO-based cuprates, irrespective of their different crystal structures. At low $p$, $T^\star$ is higher than the onset temperature of the various orders observed in underdoped cuprates, suggesting that these orders are secondary instabilities of the pseudogap phase. A linear extrapolation of $T^\star(p)$ to $p=0$ yields $T^\star(p\to 0)\simeq T_N(0)$, the N\'eel temperature for the onset of antiferromagnetic order at $p=0$, suggesting that there is a link between pseudogap and antiferromagnetism. With increasing $p$, $T^\star(p)$ extrapolates linearly to zero at $p\simeq p_{\rm c2}$, the critical doping below which superconductivity emerges at high doping, suggesting that the conditions which favour pseudogap formation also favour pairing. We also use the Nernst effect to investigate how far superconducting fluctuations extend above $T_{\rm c}$, as a function of doping, and find that a narrow fluctuation regime tracks $T_{\rm c}$, and not $T^\star$. This confirms that the pseudogap phase is not a form of precursor superconductivity.",1703.06927v2 2022-02-06,Direct observation of vortices in an electron fluid,"Vortices are the hallmarks of hydrodynamic flow. Recent studies indicate that strongly-interacting electrons in ultrapure conductors can display signatures of hydrodynamic behavior including negative nonlocal resistance, Poiseuille flow in narrow channels, and a violation of the Wiedemann-Franz law. Here we provide the first visualization of whirlpools in an electron fluid. By utilizing a nanoscale scanning superconducting quantum interference device on a tip (SQUID-on-tip) we image the current distribution in a circular chamber connected through a small aperture to an adjacent narrow current carrying strip in high-purity type-II Weyl semimetal WTe2. In this geometry, the Gurzhi momentum diffusion length and the size of the aperture determine the vortex stability phase diagram. We find that the vortices are present only for small apertures, whereas the flow is laminar (non-vortical) for larger apertures, consistent with the theoretical analysis of the hydrodynamic regime and in contrast to the expectations of ballistic transport in WTe2 at low temperatures. Moreover, near the vortical-to-laminar transition, we observe a single vortex in the chamber splitting into two vortices, a behavior that can occur only in the hydrodynamic regime and cannot be sustained by ballistic transport. These findings suggest a novel mechanism of hydrodynamic flow: instead of the commonly considered electron-electron scattering at the bulk, which becomes extremely weak at low temperatures, the spatial diffusion of charge carriers' momenta is enabled by small-angle scattering at the planar surfaces of thin pure crystals. This surface-induced para-hydrodynamics opens new avenues for exploring and utilizing electron fluidics in high-mobility electron systems.",2202.02798v1 2014-01-21,Random strain fluctuations as dominant disorder source for high-quality on-substrate graphene devices,"We have performed systematic investigations of transport through graphene on hexagonal boron nitride (hBN) substrates, together with confocal Raman measurements and a targeted theoretical analysis, to identify the dominant source of disorder in this system. Low-temperature transport measurements on many devices reveal a clear correlation between the carrier mobility $\mu$ and the width $n^*$ of the resistance peak around charge neutrality, demonstrating that charge scattering and density inhomogeneities originate from the same microscopic mechanism. The study of weak-localization unambiguously shows that this mechanism is associated to a long-ranged disorder potential, and provides clear indications that random pseudo-magnetic fields due to strain are the dominant scattering source. Spatially resolved Raman spectroscopy measurements confirm the role of local strain fluctuations, since the line-width of the Raman 2D-peak --containing information of local strain fluctuations present in graphene-- correlates with the value of maximum observed mobility. The importance of strain is corroborated by a theoretical analysis of the relation between $\mu$ and $n^*$ that shows how local strain fluctuations reproduce the experimental data at a quantitative level, with $n^*$ being determined by the scalar deformation potential and $\mu$ by the random pseudo-magnetic field (consistently with the conclusion drawn from the analysis of weak-localization). Throughout our study, we compare the behavior of devices on hBN substrates to that of devices on SiO$_2$ and SrTiO$_3$, and find that all conclusions drawn for the case of hBN are compatible with the observations made on these other materials. These observations suggest that random strain fluctuations are the dominant source of disorder for high-quality graphene on many different substrates, and not only on hexagonal boron nitride.",1401.5356v2 2018-12-07,Chemical Aspects of the Antiferromagnetic Topological Insulator MnBi$_{2}$Te$_{4}$,"Crystal growth of MnBi$_{2}$Te$_{4}$ has delivered the first experimental corroboration of the 3D antiferromagnetic topological insulator state. Our present results confirm that the synthesis of MnBi$_{2}$Te$_{4}$ can be scaled-up and strengthen it as a promising experimental platform for studies of a crossover between magnetic ordering and non-trivial topology. High-quality single crystals of MnBi$_{2}$Te$_{4}$ are grown by slow cooling within a narrow range between the melting points of Bi$_{2}$Te$_{3}$ (586 {\deg}C) and MnBi$_{2}$Te$_{4}$ (600 {\deg}C). Single crystal X-ray diffraction and electron microscopy reveal ubiquitous antisite defects in both cation sites and, possibly, Mn vacancies. Powders of MnBi$_{2}$Te$_{4}$ can be obtained at subsolidus temperatures, and a complementary thermochemical study establishes a limited high-temperature range of phase stability. Nevertheless, quenched powders are stable at room temperature and exhibit long-range antiferromagnetic ordering below 24 K. The expected Mn(II) out-of-plane magnetic state is confirmed by the magnetization, X-ray photoemission, X-ray absorption and linear dichroism data. MnBi$_{2}$Te$_{4}$ exhibits a metallic type of resistivity in the range 4.5-300 K. The compound is an n-type conductor that reaches a thermoelectric figure of merit up to ZT = 0.17. Angle-resolved photoemission experiments provide evidence for a surface state forming a gapped Dirac cone.",1812.03106v1 2018-12-19,Universal relaxation in a holographic metallic density wave phase,"In this work, we uncover a universal relaxation mechanism of pinned density waves, combining Gauge/Gravity duality and effective field theory techniques. Upon breaking translations spontaneously, new gapless collective modes emerge, the Nambu-Goldstone bosons of broken translations. When translations are also weakly broken (eg by disorder or lattice effects), these phonons are pinned with a mass $m$ and damped at a rate $\Omega$, which we explicitly compute. This contribution to $\Omega$ is distinct from that of topological defects. We show that $\Omega\simeq G m^2\Xi$, where $G$ is the shear modulus and $\Xi$ is related to a diffusivity of the purely spontaneous state. This result follows from the smallness of the bulk and shear moduli, as would be the case in a phase with fluctuating translational order. At low temperatures, the collective modes relax quickly into the heat current, so that late time transport is dominated by the thermal diffusivity. In this regime, the resistivity in our model is linear in temperature and the ac conductivity displays a significant rearranging of the degrees of freedom, as spectral weight is shifted from an off-axis, pinning peak to a Drude-like peak. These results could shed light on transport properties in cuprate high $T_c$ superconductors, where quantum critical behavior and translational order occur over large parts of the phase diagram and transport shows qualitatively similar features.",1812.08118v3 2020-06-16,Topological Dirac states in a layered telluride TaPdTe$_5$ with quasi-one-dimensional PdTe$_2$ chains,"We report the synthesis and systematic studies of a new layered ternary telluride TaPdTe5 with quasi-one-dimensional PdTe2 chains. This compound crystalizes in a layered orthorhombic structure with space group Cmcm. Analysis of its curved field-dependent Hall resistivity, using the two-band model, indicates the hole-dominated transport with a high mobility ${\mu}_h$ = 2.38 $\times$ 10$^3$ cm$^2$ V$^{-1}$ s$^{-1}$ at low temperatures. The in-plane magnetoresistance (MR) displays significant anisotropy with field applied along the crystallographic $b$ axis. The MR with the current applied along the $c$-axis is also measured in high magnetic fields up to 51.7 T. Remarkably, it follows a power-law dependence and reaches (9.5 $\times$ 10$^3$)% at 2.1 K without any signature of saturation. The De Haas-van Alphen oscillations show a small Fermi-surface pocket with a nontrivial Berry phase. The Shubnikov-de Haas (SdH) oscillations are detected at low temperatures and under magnetic fields above 28.5 T. Two effective masses $m^*$ (0.26$m_e$ and 0.41$m_e$) are extracted from the oscillatory SdH data. Our first-principles calculations unveil a topological Dirac cone in its surface states, and, in particular, the topological index indicates that TaPdTe$_5$ is a topologically nontrivial material.",2006.09070v2 2020-11-03,Pressure induced superconductivity in MnSe,"The rich phenomena in the FeSe and related compounds have attracted great interests as it provides fertile material to gain further insight into the mechanism of high temperature superconductivity. A natural follow-up work was to look into the possibility of superconductivity in MnSe. It was shown that MnP becomes superconducting with Tc ~ 1 K under pressure. We demonstrated in this work that high pressure can effectively suppress the complex magnetic characters of MnSe crystal when observed at ambient condition. MnSe under pressure is found to undergo several structural transformations: the cubic phase first partially transforms to the hexagonal phase at about 12 GPa, the crystal exhibits the coexistence of cubic, hexagonal and orthorhombic phases from 16 GPa to 30 GPa, and above 30 GPa the crystal shows a single orthorhombic phase. Superconductivity with Tc ~ 5 K was first observed at pressure ~12 GPa by magnetic measurements (~16 GPa by resistive measurements). The highest Tc is ~ 9 K (magnetic result) at ~35 GPa. Our observations suggest the observed superconductivity may closely relate to the pressure-induced structural change. However, the interface between the metallic and insulating boundaries may also play an important role to the pressure induced superconductivity in MnSe.",2011.01510v1 2020-12-24,"Structure, Electrical and Optical Properties of ITO Thin Films and their Influence on Performance of CdS/CdTe Thin-Film Solar Cells","In terms of mixing graded TiO2 and SnO2 powders by solid-state reaction method, ITO was prepared. Using electron beam gun technology, ITO films with different thicknesses were prepared. The influence of film thickness on structure, electrical and optical properties was studied. The XRD patterns were utilized to determine the structural parameters (lattice strain and crystallite size) of ITO with different thicknesses. It is observed that the average crystallite size increases as the film thickness increases, but the lattice strain decreases. SEM shows that as the film thickness increases, the grain size of ITO increases and improves. The electrical properties of ITO films with different thicknesses were measured by the standard four-point probe method. It can be seen that as the thickness of the ITO film increases from 75 nm to 325 nm, the resistivity decreases from 29x10^-4 Ohm/cm to 1.65x10^-4 Ohm/cm. This means that ITO films with lower electrical properties will be more suitable for high-efficiency CdTe solar cells. Three optical layer models (adhesive layer of the substrate/B-spline layer of ITO film/surface roughness layer) are used to calculate the film thickness with high-precision ellipsometry. In the higher T(lambda) and R(lambda) absorption regions, the absorption coefficient is determined to calculate the optical energy gap, which increases from 3.56 eV to 3.69 eV. Finally, the effects of ITO layers of various thicknesses on the performance of CdS/CdTe solar cells are also studied. When the thickness of the ITO window layer is 325 nm, Voc = 0.82 V, Jsc = 17 mA/cm2, and FF = 57.4%, the highest power conversion efficiency (PCE) is 8.6%.",2012.13086v1 2021-12-26,The thickness dependence of quantum oscillations in ferromagnetic Weyl metal SrRuO$_{3}$,"Quantum oscillations in resistivity and magnetization at high magnetic fields are a macroscopic fingerprint of the energy quantization due to the cyclotron motion of quasiparticles. In a thin Weyl semimetal, a unique thickness dependent Weyl-orbit quantum oscillation was proposed to exist, originating from a nonlocal cyclotron orbit via the electron tunneling between the top and bottom Fermi-arc surface states. Here, untwinned and high crystalline Weyl metal SrRuO$_3$ thin films with different thicknesses were grown on miscut SrTiO$_3$ (001) substrates. Magneto-transport measurements were carried out in magnetic fields up to 35 T, and quantum oscillations with different frequencies were observed and compared to the calculated band structure. In particular, we discovered a frequency $F \approx$ 30 T at low temperatures and above 3 T that corresponds to a small Fermi pocket with a light effective mass. Its oscillation amplitude appears to be at maximum for film thicknesses in a range of 10 to 20 nm, and the phase of the oscillation exhibits a systematic change with the film thickness. After isolating the well separated frequencies, the constructed Landau fan diagram shows an unusual concave downward curvature in the 1/$\mu_0H_n$-$n$ curve, where $n$ is the Landau level index. Based on the rigorous analysis of the thickness and field-orientation dependence of the quantum oscillations, the oscillation with $F \approx$ 30 T is attributed to be of surface origin, which is related to the Fermi-arc surface state originating from non-overlapping Weyl nodes projected on the film's surface plane. Those findings can be understood within the framework of the Weyl-orbit quantum oscillation effect with non-adiabatic corrections.",2112.13331v2 2022-08-04,Strong-Coupling Superconductivity with $T_c$ $\sim$ 10.8 K Induced by P Doping in the Topological Semimetal Mo$_5$Si$_3$,"By performing P doping on the Si sites in the topological semimetal Mo$_5$Si$_3$, we discover strong-coupling superconductivity in Mo$_5$Si$_{3-x}$P$_x$ (0.5 $\le$ $x$ $\le$ 2.0). Mo$_5$Si$_3$ crystallizes in the W$_5$Si$_3$-type structure with space group of $I4/mcm$ (No. 140), and is not a superconductor itself. Upon P doping, the lattice parameter $a$ decreases while $c$ increases monotonously. Bulk superconductivity is revealed in Mo$_5$Si$_{3-x}$P$_x$ (0.5 $\le$ $x$ $\le$ 2.0) from resistivity, magnetization, and heat capacity measurements. $T_c$ in Mo$_5$Si$_{1.5}$P$_{1.5}$ reaches as high as 10.8 K, setting a new record among the W$_5$Si$_3$-type superconductors. The upper and lower critical fields for Mo$_5$Si$_{1.5}$P$_{1.5}$ are 14.56 T and 105 mT, respectively. Moreover, Mo$_5$Si$_{1.5}$P$_{1.5}$ is found to be a fully gapped superconductor with strong electron-phonon coupling. First-principles calculations suggest that the enhancement of electron-phonon coupling is possibly due to the shift of the Fermi level, which is induced by electron doping. The calculations also reveal the nontrivial band topology in Mo$_5$Si$_3$. The $T_c$ and upper critical field in Mo$_5$Si$_{3-x}$P$_x$ are fairly high among pseudobinary compounds. Both of them are higher than those in NbTi, making future applications promising. Our results suggest that the W$_5$Si$_3$-type compounds are ideal platforms to search for new superconductors. By examinations of their band topologies, more candidates for topological superconductors can be expected in this structural family.",2208.02392v1 2023-05-19,Machine Learning Moment Tensor Potential for Modelling Dislocation and Fracture in L1$_0$-TiAl and D0$_{19}$-Ti$_3$Al Alloys,"Dual-phase $\gamma$-TiAl and $\alpha_2$-Ti$_{3}$Al alloys exhibit high strength and creep resistance at high temperatures. However, they suffer from low tensile ductility and fracture toughness at room temperature. Experimental studies show unusual plastic behaviour associated with ordinary and superdislocations, making it necessary to gain a detailed understanding on their core properties in individual phases and at the two-phase interfaces. Unfortunately, extended superdislocation cores are widely dissociated beyond the length scales practical for routine first-principles density-functional theory (DFT) calculations, while extant interatomic potentials are not quantitatively accurate to reveal mechanistic origins of the unusual core-related behaviour in either phases. Here, we develop a highly-accurate moment tensor potential (MTP) for the binary Ti-Al alloy system using a DFT dataset covering a broad range of intermetallic and solid solution structures. The optimized MTP is rigorously benchmarked against both previous and new DFT calculations, and unlike existing potentials, is shown to possess outstanding accuracy in nearly all tested mechanical properties, including lattice parameters, elastic constants, surface energies, and generalized stacking fault energies (GSFE) in both phases. The utility of the MTP is further demonstrated by producing dislocation core structures largely consistent with expectations from DFT-GSFE and experimental observations. The new MTP opens the path to realistic modelling and simulations of bulk lattice and defect properties relevant to the plastic deformation and fracture processes in $\gamma$-TiAl and $\alpha_2$-Ti$_{3}$Al dual-phase alloys.",2305.11825v2 2023-06-05,Imaging the Meissner effect and flux trapping in a hydride superconductor at megabar pressures using a nanoscale quantum sensor,"By directly altering microscopic interactions, pressure provides a powerful tuning knob for the exploration of condensed phases and geophysical phenomena. The megabar regime represents an exciting frontier, where recent discoveries include novel high-temperature superconductors, as well as structural and valence phase transitions. However, at such high pressures, many conventional measurement techniques fail. Here, we demonstrate the ability to perform local magnetometry inside of a diamond anvil cell with sub-micron spatial resolution at megabar pressures. Our approach utilizes a shallow layer of Nitrogen-Vacancy (NV) color centers implanted directly within the anvil; crucially, we choose a crystal cut compatible with the intrinsic symmetries of the NV center to enable functionality at megabar pressures. We apply our technique to characterize a recently discovered hydride superconductor, CeH$_9$. By performing simultaneous magnetometry and electrical transport measurements, we observe the dual signatures of superconductivity: local diamagnetism characteristic of the Meissner effect and a sharp drop of the resistance to near zero. By locally mapping the Meissner effect and flux trapping, we directly image the geometry of superconducting regions, revealing significant inhomogeneities at the micron scale. Our work brings quantum sensing to the megabar frontier and enables the closed loop optimization of superhydride materials synthesis.",2306.03122v1 2023-06-24,Exploration of strongly correlated states in SmB6 through a comparison of its two-coil pick-up response to that of Bi2Se3,"Earlier studies on the Kondo insulator SmB6 reveal the presence of a bulk Kondo insulating gap between 30 - 50 K, and the emergence of a conducting surface state only below 4 K. Here, we compare the two-coil mutual inductance pick-up response of SmB6 single crystal with that of a conventional topological insulator (TI), Bi2Se3 single crystal. From these studies we identify three distinct temperature regimes for SmB6, viz., (i) T >= T*(~ 66 K), (ii) (40 K~) T_g <= T < T*, and (iii) T < T_g. At T* in SmB6, we observe a peak in the temperature-dependent AC pickup signal which corresponds to the peak in the broad hump feature in the bulk DC susceptibility measurements and features in the resistivity measurements. A dip in the pickup signal at T_g in SmB6 correlates with the evidence for the opening of a bulk Kondo gap in transport measurements. Our study of the pickup signal in SmB6 suggests the presence of a thin (submicron order thickness) high conducting surface layer from a temperature just below T_g. In this T regime in SmB6, the pickup signal shows a distinct square root frequency (f) dependence compared to the linear f dependence found in Bi2Se3. Across all the different T regimes, distinct AC frequency dependence and scaling properties are observed. Our results suggest that above T*, weak exchange interactions cause electrons to scatter from random ion sites. Electronic correlations gradually strengthen with the onset of Kondo like hybridization, setting in from below T*, and at T_g, a strongly correlated Kondo gap opens up in the bulk of the material. The appearance of the thin high conducting surface layer is nearly coincident with the onset of bulk Kondo insulating state below T_g in SmB6.",2306.13901v1 2024-01-07,Tantalum airbridges for scalable superconducting quantum processors,"The unique property of tantalum (Ta), particularly its long coherent lifetime in superconducting qubits and its exceptional resistance to both acid and alkali, makes it promising for superconducting quantum processors. It is a notable advantage to achieve high-performance quantum processors with neat and unified fabrication of all circuit elements, including coplanar waveguides (CPW), qubits, and airbridges, on the tantalum film-based platform. Here, we propose a reliable tantalum airbridges with separate or fully-capped structure fabricated via a novel lift-off method, where a barrier layer with aluminium (Al) film is first introduced to separate two layers of photoresist and then etched away before the deposition of tantalum film, followed by cleaning with piranha solution to remove the residual photoresist on the chip. We characterize such tantalum airbridges as the control line jumpers, the ground plane crossovers and even coupling elements. They exhibit excellent connectivity, minimal capacitive loss, effectively suppress microwave and flux crosstalk and offer high freedom of coupling. Besides, by presenting a surface-13 tunable coupling superconducting quantum processor with median $T_1$ reaching above 100 $\mu$s, the overall adaptability of tantalum airbridges is verified. The median single-qubit gate fidelity shows a tiny decrease from about 99.95% for the isolated Randomized Benchmarking to 99.94% for the simultaneous one. This fabrication method, compatible with all known superconducting materials, requires mild conditions of film deposition compared with the commonly used etching and grayscale lithography. Meanwhile, the experimental achievement of non-local coupling with controlled-Z (CZ) gate fidelity exceeding 99.2% may further facilitate qLDPC codes, laying a foundation for scalable quantum computation and quantum error correction with entirely tantalum elements.",2401.03537v1 2024-04-16,A Young Super Star Cluster Powering a Nebula of Retained Massive Star Ejecta,"We suggest that ""Godzilla"", an intriguing source in the lensed Sunburst galaxy at $z=2.37$, is a young super star cluster powering a compact nebula within gravitationally trapped stellar ejecta. Employing HST photometry and spectroscopy from MUSE and X-Shooter at VLT, we infer physical and chemical properties of the cluster and nebula, finding Godzilla is young (4-6 Myr), massive ($\sim 10^{6-7}M_\odot$), a stellar metallicity $Z \simeq 0.25Z_\odot$, and has the FUV component more compact than a few pc. The nebula gas is significantly enriched with N and He, indicating stellar wind material, and has highly elevated O relative to the sub-solar stellar metallicity, which indicates entrainment of CCSNe ejecta. The high gas density $n_{\rm e} \simeq 10^{7-8}{\rm cm}^{-3}$ implies a highly pressurized intracluster environment. We propose the high pressure is due to CCSN-driven supersonic turbulence in warm, self-shielding gas, which has accumulated in the cluster center after runaway radiative cooling and is dense enough to resist removal by CCSNe. The nebula gas shows sub-solar C/O, Ne/O and Si/O values, which may reflect the CCSN element yields for initial stellar masses $>40M_\odot$. A comparison to element yield synthesis models for young star clusters shows that the gas abundance pattern is consistent with complete retention and mixture of stellar winds and CCSNe ejecta until the inferred cluster age. The O and He enhancement we find may have implications for the formation of multiple stellar populations in globular clusters, as Godzilla likely has already formed second-generation stars prior to the onset of CCSNe and evolved star winds, in order not to contradict the non-observation of O and large He enhancement in second-generation stars.",2404.10755v2 2023-02-09,Scattering-dependent transport of SrRuO3 films: From Weyl fermion transport to hump-like Hall effect anomaly,"Recent observation of quantum transport phenomena of Weyl fermions has brought much attention to 4d ferromagnetic perovskite SrRuO3 as a magnetic Weyl semimetal. Besides, the hump-like Hall effect anomaly, which might have a topological origin, has also been reported for this material. Here, we show that the emergence of such phenomena is governed by the degree of scattering determined by the defect density (Ru-deficiency- and/or interface-driven-defect scattering) and measurement temperature (phonon scattering), where the former is controlled by varying the growth conditions of the SrRuO3 films in molecular beam epitaxy as well as the film thickness. The resulting electronic transport properties can be classified into three categories: clean, intermediate, and dirty regimes. The transport of Weyl fermions emerges in the clean regime, whereas that of topologically trivial conduction electrons in the ferromagnetic metal state prevail in the intermediate and dirty regimes. In the clean and intermediate regimes, anomalous Hall resistivity obeys a scaling law incorporating the intrinsic Karplus-Luttinger (Berry phase) and extrinsic side-jump mechanisms. The hump-like Hall effect anomaly is observed only in the dirty regime, which is contrary to the scaling law between anomalous Hall resistivity and longitudinal resistivity. Hence, we conclude that this anomaly is not inherent to the material and does not have a topological origin. We also provide defect- and temperature-dependent transport phase diagrams of stoichiometric SrRuO3 and Ru-deficient SrRu0.7O3 where the appearance of Weyl fermions and hump-like Hall effect anomaly are mapped. These diagrams may serve as a guideline for designing SrRu1-xO3-based spintronic and topological electronic devices.",2302.04568v1 2024-02-29,"Magnetism, heat capacity and electronic structure of EuCd$_2$P$_2$ in view of its colossal magnetoresistance","The mechanism of the peculiar transport properties around the magnetic ordering temperature of semiconducting antiferromagnetic EuCd$_2$P$_2$ is not yet understood. With a huge peak in the resistivity observed above the N\'eel temperature, $T_{\rm N}=10.6\,\rm K$, it exhibits a colossal magnetoresistance effect. Recent reports on observations of ferromagnetic contributions above $T_{\rm N}$ as well as metallic behavior below this temperature have motivated us to perform a comprehensive characterization of this material, including its resistivity, heat capacity, magnetic properties and electronic structure. Our transport measurements revealed quite different temperature dependence of resistivity with the maximum at $14\,\rm K$ instead of previously reported $18\,\rm K$. Low-field susceptibility data support the presence of static ferromagnetism above $T_{\rm N}$ and show a complex behavior of the material at small applied magnetic fields. Namely, signatures of reorientation of magnetic domains are observed up to $T=16\,\rm K$. Our magnetization measurements indicate a magnetocrystalline anisotropy which also leads to a preferred alignment of the magnetic clusters above $T_{\rm N}$. The momentum-resolved photoemission experiments at temperatures from $24\,\rm K$ down to $2.5\,\rm K$ indicate the permanent presence of a fundamental band gap without change of the electronic structure when going through $T_N$ that is in contradiction with previous results. We performed \textit{ab initio} band structure calculations which are in good agreement with the measured photoemission data when assuming an antiferromagnetic ground state. Calculations for the ferromagnetic phase show a much smaller bandgap, indicating the importance of possible ferromagnetic contributions for the explanation of the colossal magnetoresistance effect in the related EuZn$_2$P$_2$.",2402.18911v1 2023-01-14,Discovery of 2D materials using Transformer Network based Generative Design,"Two-dimensional (2D) materials have wide applications in superconductors, quantum, and topological materials. However, their rational design is not well established, and currently less than 6,000 experimentally synthesized 2D materials have been reported. Recently, deep learning, data-mining, and density functional theory (DFT)-based high-throughput calculations are widely performed to discover potential new materials for diverse applications. Here we propose a generative material design pipeline, namely material transformer generator(MTG), for large-scale discovery of hypothetical 2D materials. We train two 2D materials composition generators using self-learning neural language models based on Transformers with and without transfer learning. The models are then used to generate a large number of candidate 2D compositions, which are fed to known 2D materials templates for crystal structure prediction. Next, we performed DFT computations to study their thermodynamic stability based on energy-above-hull and formation energy. We report four new DFT-verified stable 2D materials with zero e-above-hull energies, including NiCl$_4$, IrSBr, CuBr$_3$, and CoBrCl. Our work thus demonstrates the potential of our MTG generative materials design pipeline in the discovery of novel 2D materials and other functional materials.",2301.05824v1 2014-05-15,Effect of high pressure annealing on the normal state transport of LaO0.5F0.5BiS2,"We study normal state electrical, thermoelectrical and thermal transport in polycrystalline BiS2-based compounds, which become superconducting by F doping on the O site. In particular we explore undoped LaOBiS2 and doped LaO0.5F0.5BiS2 samples, prepared either with or without high pressure annealing, in order to evidence the roles of doping and preparation conditions. The high pressure annealed sample exhibits room temperature values of resistivity ro around 5 mohmcm, Seebeck coefficient S around -20 microV/K and thermal conductivity k around 1.5 W/Km, while the Hall resistance RH is negative at all temperatures and its value is -10-8 m3/C at low temperature. The sample prepared at ambient pressure exhibits RH positive in sign and five times larger in magnitude, and S negative in sign and slightly smaller in magnitude. These results reveal a complex multiband evolution brought about by high pressure annealing. In particular, the sign inversion and magnitude suppression of RH, indicating increased electron-type carrier density in the high pressure sample, may be closely related to previous findings about change in lattice parameters and enhancement of superconducting Tc by high pressure annealing. As for the undoped sample, it exhibits the 10 times larger resistivity, 10 times larger |S| and 10 times larger |RH| than its doped counterpart, consistently with its insulating nature. Our results point out the dramatic effect of preparation conditions in affecting charge carrier density as well as structural, band and electronic parameters in these systems.",1405.3832v2 2021-09-05,On the design of particle filters inspired by animal noses,"Passive filtering is a common strategy used to reduce airborne disease transmission and particulate contaminants in buildings and individual covers. The engineering of high-performance filters with relatively low flow resistance but high virus- or particle-blocking efficiency is a nontrivial problem of paramount relevance, as evidenced in the variety of industrial filtration systems and the worldwide use of face masks. In this case, standard N95-level covers have high virus-blocking efficiency, but they can cause breathing discomfort. Next-generation industrial filters and masks should retain sufficiently small droplets and aerosols while having low resistance. We introduce a novel 3D printable particle filter inspired by animals' complex nasal anatomy. Unlike standard random-media-based filters, the proposed concept relies on equally spaced channels with tortuous airflow paths. These two strategies induce distinct effects: a reduced resistance and a high likelihood of particle trapping by altering their trajectories with tortuous paths and induced local flow instability. The structures are tested for pressure drop and particle filtering efficiency over a wide range of airflow rates. We have also cross-validated the observed efficiency through numerical simulations. The designed filters exhibit a lower pressure drop than the commercial mask and air filters (N95, surgical, and high-efficiency particulate air (HEPA)). The concept provides a new approach to developing scalable, flexible, high-efficiency air filters for various engineering applications.",2109.08018v1 1997-09-27,"Low-temperature electrical transport and double exchange in La(Pb,Ca)MnO","The resistivity in the ferromagnetic state of flux-grown La_{2/3}(Pb,Ca)_{1/3}MnO_3 single crystals, measured in magnetic fields up to 7 T, reveals a strong quadratic temperature dependence at and above 50 K. At lower temperatures, this contribution drops precipitously leaving the resistivity essentially temperature independent below 20 K. The Seebeck coefficient also reflects a change of regime at the same temperature. We attribute this behavior to a cut-off of single magnon scattering processes at long wavelengths due to the polarized bands of a double-exchange ferromagnet.",9709305v3 1998-01-07,Theory of the Resistive Transition in Overdoped $Tl_2Ba_2CuO_{6+x}$: Implications for the angular dependence of the quasiparticle scattering rate in High-$T_c$ superconductors,"We show that recent measurements of the magnetic field dependence of the magnetization, specific heat and resistivity of overdoped $T_c \sim 17K$ $Tl_{2}Ba_{2}CuO_{6+\delta}$ in the vicinity of the superconducting $H_{c2}$ imply that the vortex viscosity is anomalously small and that the material studied is inhomogeneous with small, a few hundred $\AA$, regions in which the local $T_{c}$ is much higher than the bulk $T_{c}$. The anomalously small vortex viscosity can be derived from a microscopic model in which the quasiparticle lifetime varies dramatically around the Fermi surface, being small everywhere except along the zone diagonal (``cold spot''). We propose experimental tests of our results.",9801059v1 1998-08-25,P-wave Pairing and Colossal Magnetoresistance in Manganese Oxides,"We point out that the existing experimental data of most manganese oxides show the {\sl frustrated} p-wave superconducting condensation in the ferromagnetic phase in the sense that the superconducting coherence is not long enough to cover the whole system. The superconducting state is similar to the $A_{1}$ state in superfluid He-3. The sharp drop of resistivity, the steep jump of specific heat, and the gap opening in tunneling are well understood in terms of the p-wave pairing. In addition, colossal magnetoresistance (CMR) is naturally explained by the superconducting fluctuations with increasing magnetic fields. The finite resistivity may be due to some magnetic inhomogeneities. This study leads to the possibility of room temperature superconductivity.",9808275v1 1998-10-30,"Hall Effect of La2/3(Ca,Pb)1/3MnO3 Single Crystals near the Critical Temperature","The Hall resistivity rho_{xy} of a La_{2/3}(Ca,Pb)_{1/3}MnO_3 single crystal has been measured as a function of temperature and field. The overall behavior is similar to that observed previously in thin-films. At 5 K, rho_{xy} is positive and linear in field, indicating that the anomalous contribution $R_S$ is negligible. However, the effective carrier density in a free electron model is n_{eff}=2.4 holes/Mn, even larger than the 0.85-1.9 holes/Mn reported for thin-films and far larger than the 0.33 holes/Mn expected from the doping level. As temperature increases, a strong, negative contribution to rho_{xy} appears, that we ascribe to R_S. Using detailed magnetization data, we separate the ordinary (\propto B) and anomalous (\propto M) contributions. Below T_C, R_S \propto rho_{xx}, indicating that magnetic skew scattering is the dominant mechanism in the metallic ferromagnetic regime. At and above the resistivity-peak temperature, we find that rho_{xy}/rho_{xx}M is a constant, independent of temperature and field. This implies that the anomalous Hall coefficient is proportional to the magnetoresistance. A different explanation based on two fluid model is also presented.",9810410v1 1998-11-28,Negative Differential Resistance in the Scanning Tunneling Spectroscopy of Organic molecules,"The conductance-voltage spectrum of molecular nanostructures measured by scanning tunneling spectroscopy (STS) is generally assumed to reflect the local density of states of the molecule. This excludes the possibility of observing negative differential resistance (NDR). We report here the observation of NDR in the scanning tunneling microscope (STM) current-voltage (I-V) characteristics of self-assembled monolayer (SAM) of 4-p-Terphenylthiol molecules on gold substrate measured using a platinum probe. We argue that the NDR arises from narrow structures in the local density of states at the tip apex atom and show that depending on the electrostatic potential profile across the system, NDR could be observed in one or both bias directions.",9811402v1 1998-12-27,Field Induced Transition from Metal to Insulator in the CMR Manganites,"The gigantic reduction of the electric resistivity under the applied magnetic field, CMR effect, is now widely accepted to appear in the vicinity of the insulator to metal transition of the perovskite manganites. Recently, we have discovered the first order transition from ferromagnetic metal to insulator in $\rm La_{0.88}Sr_{0.12}MnO_3$ of the CMR manganite. This phase transition induces the tremendous increase of the resistivity under the external magnetic field just near above the phase transition temperature. We report here fairly detailed results from the systematic experiments including neutron and synchrotron X-ray scattering studies.",9812404v1 1999-01-25,Influence of Cu on spin-polaron tunneling in the ferromagnetic state of La(2/3)Ca(1/3)Mn(1-x)Cu(x)O(3) from the resistivity data,"Nearly a 50% decrease of resistivity \rho (T,x) due to just 4% Cu doping on the Mn site of La(2/3)Ca(1/3)Mn(1-x)Cu(x)O(3) is observed. Attributing the observed phenomenon to the substitution induced decrease of the spin polaron energy E_s(x) below the Curie point T_C(x)=T_C(0)(1-x), all data are found to be well fitted by the nonthermal coherent tunneling expression \rho (T,x) = \rho_0*exp(-\gamma M^2(T,x)) assuming M(T,x)=M_R(x)+M_0(x)*tanh{\sqrt{[T_C(x)/T]^2-1}} for the magnetization in the ferromagnetic state. The best fits through all the data points yield M_0(x)= \sqrt(1-x)M_0(0), M_R(x)=\sqrt(x)M_0(0), and E_s(x)=E_s(0)(1-x)^4 for the Cu induced modifications of the Mn spins dominated zero-temperature spontaneous magnetization, the residual paramagnetic contribution, and spin-polaron energy, respectively, with E_s(0)=0.12 eV.",9901263v1 1999-03-03,c-axis Tunneling in Nb/Au/YBaCuO Structures,"We present the experimental results for Nb/Au/YBaCuO structures, in which the current flows along (001) direction of YBaCuO film. The theoretical evaluations show, that at the experimental values of the Au/YBaCuO interface transparency, determined from the interface resistance D~10^-6, the critical current of the structure is of the fluctuation order of magnitude due to the sharp decrease of the amplitude potential of the superconducting carriers on this interface. Obtained I-V-curves could be interpreted in terms of contact between d-type pairing superconductor or gapless isotropic superconductor with normal metal. No critical current was observed for investigated structures with characteristic interface resistance RnS~10^-6 Ohm cm^2, 2 orders of magnitude lower, than for known experimental data. PACS: 74.50.+r, 74.72.Bk",9903065v1 1999-03-15,Metal-insulator transition in CMR materials,"We report on resistivity measurements in La$_{0.67}$Ca$_{0.33}$MnO$_{3}$ and Nd$_{0.7}$Sr$_{0.3}$MnO$_{3}$ thin films in order to elucidate the underlying mechanism for the CMR behavior. The experimental results are analyzed in terms of quantum phase transition ideas to study the nature of the metal-insulator transition in manganese oxides. Resistivity curves as functions of magnetization for various temperatures show the absence of scaling behavior expected in a continuous quantum phase transition, which leads us to conclude that the observed metal-insulator transition is most likely a finite temperature crossover phenomenon.",9903238v2 2000-01-06,Time Dependent Effects and Transport Evidence for Phase Separation in La_{0.5}Ca_{0.5}MnO_{3},"The ground state of La_{1-x}Ca_{x}MnO_{3} changes from a ferromagnetic metallic to an antiferromagnetic charge-ordered state as a function of Ca concentration at x ~ 0.50. We present evidence from transport measurements on a sample with x = 0.50 that the two phases can coexist, in agreement with other observations of phase separation in these materials. We also observe that, by applying and then removing a magnetic field to the mainly charge-ordered state at some temperatures, we can ""magnetically anneal"" the charge order, resulting in a higher zero-field resistivity. We also observe logarithmic time dependence in both resistivity and magnetization after a field sweep at low temperatures.",0001064v1 2000-02-14,Transition Temperature and Magnetoresistance in Double-Exchange Compounds with Moderate Disorder,"We develop a variational mean-field theory of the ferromagnetic transition in compounds like Lanthanum-Manganite within the framework of the Double-Exchange Model supplemented by modest disorder. We obtain analytical expressions for the transition temperature, its variation with the valence electron-density and its decrease with disorder. We derive an expression for the conductivity for both the paramagnetic and the ferromangetic metallic phases, and study its dependence on the temperature and magnetic field. A simple relation between the resistivity in the ferromagnetic phase and the spontaneous magnetization is found. Our results are in a good agreement with the experimental data on transition temperatures and resistivity in the manganite compounds with relatively small disorder. We comment on the effects of increased disorder.",0002191v1 2000-03-11,Effect of γ-irradiation on superconducting transition temperature and resistive transition in polycrystalline YBa_{2}Cu_{3}O_(7-δ),"A bulk polycrystalline sample of YBa_(2)Cu_(3)O_(7-\delta) (\delta \approx 0.1) has been irradiated by \gamma-rays with ^{60}Co source. Non-monotonic behavior of T_{c} with increasing irradiation dose \Phi (up to 220 MR) is observed: T_{c} decreases at low doses (\Phi < 50 MR) from initial value (\approx 93 K) by about 2 K and then rises, forming a minimum. At higher doses (\Phi > 120 MR) T_{c} goes down again. The temperature width of resistive transition increases rather sharply with dose below 75 MR and drops somewhat at higher dose. The results observed are discussed, taking into account the granular structure of sample studied and the influence of \gamma-rays on intergrain Josephson coupling.",0003192v1 2000-06-07,Step-wise Behavior of Vortex-Lattice Melting Transition in Tilted Magnetic Fields in Single Crystals Bi2Sr2CaCu2O8+d,"The vortex lattice melting transition in single crystals Bi2Sr2CaCu2O8+d was studied by the in-plane resistivity measurements in magnetic fields tilted away from the c-axis to the ab-plane. In order to avoid the surface barrier effect which hinders the melting transition in the conventional transport measurements, we used the Corbino geometry of electric contacts. For the first time, the complete Hc-Hab phase diagram of the melting-transition in Bi2Sr2CaCu2O8+d is obtained. The c-axis melting field component Hc-melt exhibits the novel, step-wise dependence on the in-plane magnetic fields Hab which is discussed on the base of the crossing vortex lattice structure. The sharp change of resistance behavior observed near the ab-plane suggests transformation from first-order to second-order phase transition.",0006095v1 2000-08-07,Large two-level magnetoresistance effect in doped manganite grain boundary junctions,"We performed a systematic analysis of the tunneling magnetoresistance (TMR) effect in single grain boundary junctions formed in epitaxial La(2/3)Ca(1/3)MnO(3) films deposited on SrTiO(3) bicrystals. For magnetic fields H applied parallel to the grain boundary barrier, an ideal two-level resistance switching behavior with sharp transitions is observed with a TMR effect of up to 300% at 4.2 K and still above 100% at 77 K. Varying the angle between H and the grain boundary results in differently shaped resistance vs H curves. The observed behavior is explained within a model of magnetic domain pinning at the grain boundary interface.",0008105v1 2000-10-20,"Composite Spin Waves, Quasi-Particles and Low Temperature resistivity in Double Exchange Systems","We make a quantum description of the electron low temperature properties of double exchange materials. In these systems there is a strong coupling between the core spin and the carriers spin. This large coupling makes the low energy spin waves to be a combination of ion and electron density spin waves. We study the form and dispersion of these composite spin wave excitations. We also analyze the spin up and down spectral functions of the temperature dependent quasi-particles of this system. Finally we obtain that the thermally activated composite spin waves renormalize the carriers effective mass and this gives rise to a low temperature resistivity scaling as T ^{5/2}.",0010312v1 2000-12-13,Phase-coherence transition in granular superconductors with $π$ junctions,"We study the three-dimensional XY-spin glass as a model for the resistive behavior of granular superconductors containing a random distribution of $\pi$ junctions, as in high-$T_c$ superconducting materials with d-wave symmetry. The $\pi$ junctions leads to quenched in circulating currents (chiralities) and to a chiral-glass state at low temperatures, even in the absence of an external magnetic field. Dynamical simulations in the phase representation are used to determine the nonlinear current-voltage characteristics as a function of temperature. Based on dynamic scaling analysis, we find a phase-coherence transition at finite temperature below which the linear resistivity should vanish and determine the corresponding critical exponents. The results suggest that the phase and chiralities may order simultaneously for decreasing temperatures into a superconducting chiral-glass state.",0012238v1 2000-12-19,Resistance Spikes at Transitions between Quantum Hall Ferromagnets,"We report a new manifestation of first-order magnetic transitions in two-dimensional electron systems. This phenomenon occurs in aluminum arsenide quantum wells with sufficiently low carrier densities and appears as a set of hysteretic spikes in the resistance of a sample placed in crossed parallel and perpendicular magnetic fields, each spike occurring at the transition between states with different partial magnetizations. Our experiments thus indicate that the presence of magnetic domains at the transition starkly increases dissipation, an effect also suspected in other ferromagnetic materials. Analysis of the positions of the transition spikes allows us to deduce the change in exchange-correlation energy across the magnetic transition, which in turn will help improve our understanding of metallic ferromagnetism.",0012367v1 2001-01-30,Stress-induced metallic behavior under magnetic field in Pr$_{1-x}$Ca$_{x}$MnO$_{3}$ (x = 0.5 and 0.4) thin films,"We have investigated the role of the stress-induced by the presence of the substrate in thin films of colossal magnetoresistive manganites on structural, resistive and magnetic properties. Because of the strong coupling between the small structural distortions related to the charge-ordering (CO) and the resistive properties, the presence of the substrate prevents the full developpement of the charge ordering in Pr$_{0.5}$Ca$_{0.5}$MnO$_{3}$, especially in the very thin films. For thicker films, the CO state exists, but is not fully developped. Correlatively, the magnetic field which is necessary to suppress the CO is decreased drastically from 25 Tesla to about 5 Tesla on SrTiO$_{3}$ substrates. We have also investigated the influence of the doping level by studying the case of Pr$_{0.6}$Ca$_{0.4}$MnO$_{3}$.",0101448v1 2001-04-18,Electron Transport in Diborides: Observation of Superconductivity in ZrB2,"We report on syntheses and electron transport properties of polycrystalline samples of diborides (AB2) with different transition metals atoms (A=Zr,Nb,Ta). The temperature dependence of resistivity, \rho(T), and ac susceptibility of these samples reveal superconducting transition of ZrB2 with Tc=5.5 K, while NbB2 and TaB2 have been observed nonsuperconducting up to 0.37 K. Hc2(T) is linear in temperature below Tc, leading to a rather low Hc2(0)= 0.1 T. At T close to Tc, Hc2(T) demonstrates a downward curvature. We conclude that these diborides as well as MgB2 samples behaves like a simple metals in the normal state with usual Bloch-Gr\""uneisen temperature dependence of resistivity and with Debye temperatures: 280 K, 460 K and 440 K, for ZrB2, NbB2 and MgB2, respectively, rather than T^2 and T^3 as previously reported for MgB2.",0104323v1 2001-05-02,In-plane Hall effect in c-axis-oriented MgB2 thin films,"We have measured the longitudinal resistivity and the Hall resistivity in the ab-plane of highly c-axis-oriented MgB2 thin films. In the normal state, the Hall coefficient (R_H) behaves as R_H ~ T with increasing temperature (T) up to 130 K and then deviates from that linear T-dependence at higher temperatures. The T^2 dependence of the cotangent of the Hall angle is only observed above 130 K. The mixed-state Hall effect reveals no sign anomaly over a wide range of current densities from 10^2 to 10^4 A/cm^2 and for magnetic fields up to 5 T.",0105024v2 2001-05-04,A New Method of Probing the Phonon Mechanism in Superconductors including MgB$_{2}$,"Weak localization has a strong influence on both the normal and superconducting properties of metals. In particular, since weak localization leads to the decoupling of electrons and phonons, the temperature dependence of resistance (i.e., $\lambda_{tr}$) is decreasing with increasing disorder, as manifested by Mooij's empirical rule. In addition, Testardi's universal correlation of $T_{c}$ (i.e., $\lambda$) and the resistance ratio (i.e., $\lambda_{tr}$) follows. This understanding provides a new means to probe the phonon mechanism in superconductors including MgB$_{2}$. The merits of this method are its applicability to any superconductors and its reliability because the McMillan's electron-phonon coupling constant $\lambda$ and $\lambda_{tr}$ change in a broad range, from finite values to zero, due to weak localization. Karkin et al's preliminary data of irradiated MgB$_{2}$ show the Testardi correlation, indicating that the dominant pairing mechanism in MgB$_{2}$ is the phonon-mediated interaction.",0105091v1 2002-01-25,Degradation of LaMnO{3-y} surface layer in LaMnO{3-y}/ metal interface,"We report electrical measurements showing the degradation processes of LaMnO$_{3-y}$ (LaMnO) in LaMnO/normal metal interface in both point contact and planar-type junctions. Immediately after the preparation of the interface, the degradation process was followed by measuring the evolution of the junction resistance versus time. This process is characterized by the appearance of a second maximum in the resistance vs. temperature (R-T) dependence at temperatures lower than the Curie temperature T$_c$, at which the metal-insulator transition occurs in the bulk. These effects are explained in terms of the formation of a depleted interface layer in LaMnO caused by an out-diffusion of oxygen from the manganite surface to the normal metal. This assumption is confirmed by XPS measurement. Similar results on LaSrMnO$_{3-y}$ interfaces are also obtained.",0201460v1 2002-02-06,Thermoelectric properties of the brownmillerite oxide Ca_{2-y}La_yCo_{2-x}Al_xO_5,"We prepared the brownmillerite oxide Ca_{2-y}La_yCo_{2-x}Al_xO_5, and found that it was an n-type conductor. The thermopower and the resistivity of the single crystal are -90 microV/K and 68 mOhm cm along the ab direction at 440 K, which suggest relatively good thermoelectrical properties, compared with other transition-metal oxides. Their temperature dependences are of activation type, and the activation energies are 0.2 eV for the resistivity and 0.04 eV for the thermopower. These energies differ by one order in magnitude, which implies that a polaron dominates the charge transport. A sign of the thermopower of the polycrystals changes from negative to positive at 500 K, indicating that holes are excited thermally to decrease the magnitude of thermopower.",0202087v1 2002-04-29,Concentration of Charge Carriers and Anomalous Gap Parameter in the Normal State of High-$T_c$ Superconductors,"Fermi-Dirac statistics has been utilized by introducing the average ionization energy ($E_I$) as an additional anomalous energy gap in order to derive the two-dimensional concentration of charge carriers and the phenomenological resistivity model for the superconducting polycrystalline materials. The best fitted values of $E_I$ and the charge carriers' concentration ranges in the vicinity of 4 to 9 meV and 10$^{16}$ m$^{-2}$ respectively for the superconducting single crystal samples and polycrystalline compounds synthesized with various compositions via solid-state reactions. The phenomenological resistivity model is further redefined here based on the gapless nature of charge-carriers' dynamics within the Cu-O$_2$ planes that corresponds to anomalous Fermi liquid behavior, which is in accordance with the nested Fermi liquid theory.",0204601v1 2002-08-09,Quasi-one-dimensional superconductivity above 300 K and quantum phase slips in individual carbon nanotubes,"A great number of the existing data for electrical transport, the Altshuler Aronov Spivak and Aharonov Bohm effects, as well as the tunneling spectra of individual carbon nanotubes can be well explained by theories of the quantum phase slips in quasi-one-dimensional superconductors. The existing data consistently suggest that the mean-field superconducting transition temperature T_{c0} in both single-walled and multi-walled carbon nanotubes could be higher than 600 K. The quantum phase slip theories naturally explain why the on-tube resistances in the closely packed nanotube bundles or in the individual multi-walled nanotubes with large diameters approach zero at room temperature, while a single tube with a small diameter has a substantial resistance.",0208198v4 2002-08-13,Characterization of one-dimensional quantum channels in InAs/AlSb,"We report the magnetoresistance characteristics of one-dimensional electrons confined in a single InAs quantum well sandwiched between AlSb barriers. As a result of a novel nanofabrication scheme that utilizes a 3nm-shallow wet chemical etching to define the electrostatic lateral confinement, the system is found to possess three important properties: specular boundary scattering, a strong lateral confinement potential, and a conducting channel width that is approximately the lithography width. Ballistic transport phenomena, including the quenching of the Hall resistance, the last Hall plateau, and a strong negative bend resistance, are observed at 4K in cross junctions with sharp corners. In a ring geometry, we have observed Aharonov-Bohm interference that exhibits characteristics different from those of the GaAs counterpart due to the ballistic nature of electron transport and the narrowness of the conducting channel width.",0208265v1 2002-08-27,Anomalous Hall Effect of Calcium-doped Lanthanum Cobaltite Films,"The Hall resistivity, magnetoresistance, and magnetization of La_{1-x}Ca_{x}CoO_{3} epitaxial films with x between 0.25 and 0.4 grown on lanthanum aluminate were measured in fields up to 7 T. The x=1/3 film, shows a reentrant metal insulator transition. Below 100 K, the x=1/3 and 0.4 films have significant coercivity which increases with decreasing temperature. At low temperature the Hall resistivity remains large and essentially field independent in these films, except for a sign change at the coercive field that is more abrupt than the switching of the magnetization. A unique magnetoresistance behavior accompanies this effect. These results are discussed in terms of a percolation picture and the mixed spin state model for this system. We propose that the low-temperature Hall effect is caused by spin-polarized carriers scattering off of orbital disorder in the spin-ordered clusters.",0208530v1 2003-01-24,Semiconductive and Photoconductive Properties of the Single Molecule Magnets Mn$_{12}$-Acetate and Fe$_8$Br$_8$,"Resistivity measurements are reported for single crystals of Mn$_{12}$-Acetate and Fe$_8$Br$_8$. Both materials exhibit a semiconductor-like, thermally activated behavior over the 200-300 K range. The activation energy, $E_a$, obtained for Mn$_{12}$-Acetate was 0.37 $\pm$ 0.05 eV, which is to be contrasted with the value of 0.55 eV deduced from the earlier reported absorption edge measurements and the range of 0.3-1 eV from intramolecular density of states calculations, assuming $2E_a$= $E_g$, the optical band gap. For Fe$_8$Br$_8$, $E_a$ was measured as 0.73 $\pm$ 0.1 eV, and is discussed in light of the available approximate band structure calculations. Some plausible pathways are indicated based on the crystal structures of both lattices. For Mn$_{12}$-Acetate, we also measured photoconductivity in the visible range; the conductivity increased by a factor of about eight on increasing the photon energy from 632.8 nm (red) to 488 nm (blue). X-ray irradiation increased the resistivity, but $E_a$ was insensitive to exposure.",0301497v1 2003-02-12,Avoided Antiferromagnetic Order and Quantum Critical Point in CeCoIn$_5$,"We measured specific heat and resistivity of heavy fermion CeCoIn5 between the superconducting critical field $H_{c2} = 5 T$ and 9 T, with field in the [001] direction, and at temperatures down to 50mK. At 5T the data show Non Fermi Liquid behavior down to the lowest temperatures. At field above 8T the data exhibit crossover from the Fermi liquid to a Non Fermi Liquid behavior. We analyzed the scaling properties of the specific heat, and compared both resistivity and the specific heat with the predictions of a spin-fluctuation theory. Our analysis leads us to suggest that the NFL behavior is due to incipient antiferromagnetism (AF) in CeCoIn5, with the quantum critical point in the vicinity of the $H_{c2}$. Below $H_{c2}$ the AF phase which competes with the paramagnetic ground state is superseded by the superconducting transition.",0302226v1 2003-02-21,Anomalous Hall Effect and Magnetoresistance of SrFe1-xCoxO3-d,"Transport and magnetic studies on polycrystalline samples of SrFe1-xCoxO3-d have been carried out to investigate the relationship between the magnetic structure and the anomalous Hall resistivity rH. The hysteretic behavior of the magnetization observed in the measurements with varying temperature T up and then down after zero field cooling indicates that the system has the reentrant spin-glass phase, which is supported by the increasing width of the magnetic reflections observed by neutron diffraction with decreasing T below the Curie temperature TC. Detailed analyses of the observed Hall resistivity rH indicate that the anomalous Hall coefficient exhibits unusual behavior in the reentrant spin-glass phase. The magnetic field (H)- and T-dependence of the magnetoresistance of the present system can be understood by a spin dependent tunneling model.",0302436v1 2003-02-24,Spin-wave scattering at low temperatures in manganite films,"The temperature $T$ and magnetic field $H$ dependence of the resistivity $\rho$ has been measured for La$_{0.8-y}$Sr$_{0.2}$MnO$_{3}$ (y=0 and 0.128) films grown on (100) SrTiO$_{3}$ substrates. The low-temperature $\rho$ in the ferromagnetic metallic region follows well $\rho (H,T)=\rho _{0}(H)+A(H)\omega_{s}/\sinh (\hbar \omega_{s}/2k_{B}T)+B(H)T^{7/2}$ with $\rho _{0}$ being the residual resistivity. We attribute the second and third term to small-polaron and spin-wave scattering, respectively. Our analysis based on these scattering mechanisms also gives the observed difference between the metal-insulator transition temperatures of the films studied. Transport measurements in applied magnetic field further indicate that spin-wave scattering is a key transport mechanism at low temperatures.",0302486v1 2003-04-07,Thickness dependence of the properties of epitaxial MgB2 thin films grown by hybrid physical-chemical vapor deposition,"We have studied the effect of deposition rate and layer thickness on the properties of epitaxial MgB2 thin films grown by hybrid physical-chemical vapor deposition on 4H-SiC substrates. The MgB2 film deposition rate depends linearly on the concentration of B2H6 in the inlet gas mixture. We found that the superconducting and normal-state properties of the MgB2 films are determined by the film thickness, not by the deposition rate. When the film thickness was increased, the transition temperature, Tc, increased and the residual resistivity, rho0, decreased. Above about 300 nm, a Tc of 41.8 K, a rho0 of 0.28 mikroOhm.cm, and a residual resistance ratio RRR of over 30 were obtained. These values represent the best MgB2 properties reported thus far.",0304164v1 2003-06-05,Variable-range-hopping conductivity of half-doped bilayer manganite LaSr$_{2}$Mn$_{2}$O$_{7}$,"We report measurements of in-plane $\rho_{ab}$ and out-of-plane $\rho_{c}$ resistivities on a single crystal of the half-doped bilayer manganite LaSr$_{2}$Mn$_{2}$O$_{7}$. In the temperature $T$ range 220 to 300 K, the resistive anisotropy $\rho_{c}/\rho_{ab}=A+B/T$ ($A$ and $B$ constants), which provides evidence for the variable-range-hopping conduction in the presence of a Coulomb gap. This hopping mechanism also accounts for the quadratic magnetic field $H$ and $\sin^{2}\phi$ dependences of the negative magnetoresistivity $\ln [\rho_{i}(T,H,\phi)/\rho_{i}(T,H=0)]$ ($i=ab,c$), where $\phi$ is the in-plane angle between the magnetic field and the current.",0306133v1 2003-06-11,"Enhanced electrical resistivity before Néel order in the metals, RCuAs$_2$ (R= Sm, Gd, Tb and Dy","We report an unusual temperature (T) dependent electrical resistivity($\rho$) behavior in a class of ternary intermetallic compounds of the type RCuAs$_2$ (R= Rare-earths). For some rare-earths (Sm, Gd, Tb and Dy) with negligible 4f-hybridization, there is a pronounced minimum in $\rho$(T) far above respective N\'eel temperatures (T$_N$). However, for the rare-earths which are more prone to exhibit such a $\rho$(T) minimum due to 4f-covalent mixing and the Kondo effect, this minimum is depressed. These findings, difficult to explain within the hither-to-known concepts, present an interesting scenario in magnetism.",0306266v1 2003-07-14,"Interplay between disorder, quantum and thermal fluctuations in ferromagnetic alloys: The case of UCu2Si(2-x)Ge(x)","We consider, theoretically and experimentally, the effects of structural disorder, quantum and thermal fluctuations in the magnetic and transport properties of certain ferromagnetic alloys.We study the particular case of UCu2Si(2-x)Ge(x). The low temperature resistivity, rho(T,x), exhibits Fermi liquid (FL) behavior as a function of temperature T for all values of x, which can be interpreted as a result of the magnetic scattering of the conduction electrons from the localized U spins. The residual resistivity, rho(0,x), follows the behavior of a disordered binary alloy. The observed non-monotonic dependence of the Curie temperature, Tc(x), with x can be explained within a model of localized spins interacting with an electronic bath whose transport properties cross-over from ballistic to diffusive regimes. Our results clearly show that the Curie temperature of certain alloys can be enhanced due to the interplay between quantum and thermal fluctuations with disorder.",0307328v2 2003-10-20,Studies of Current-Driven Excitations in Co/Cu/Co Trilayer Nanopillars,"We measure the dynamic resistance of a Co/Cu/Co trilayer nanopillar at varied magnetic field $H$ and current $I$. The resistance displays the usual behavior, almost symmetric in $H$, both when magnetization switching is hysteretic at small $I,H$, and reversible at larger $I,H$. We show differences in the $I,H$ magnetization stability diagram measured by holding $I$ fixed and varying $H$ and vice versa. We also show how the peak in $dV/dI$ associated with telegraph noise in the reversible switching regime, is calculated from the telegraph noise variations with $I$. Lastly, we show data for a similar sample that displays behavior asymmetric in $H$, and a negative reversible switching peak instead of a usual positive one.",0310472v1 2003-11-17,The Normal State Resistivity of Grain Boundaries in YBa2Cu3O7-delta,"Using an optimized bridge geometry we have been able to make accurate measurements of the properties of YBa2Cu3O7-delta grain boundaries above Tc. The results show a strong dependence of the change of resistance with temperature on grain boundary angle. Analysis of our results in the context of band-bending allows us to estimate the height of the potential barrier present at the grain boundary interface.",0311386v1 2004-02-09,Molecular electronics exploiting sharp structure in the electrode density-of-states. Negative differential resistance and Resonant Tunneling in a poled molecular layer on Al/LiF electrodes,"Density-functional calculations are used to clarify the role of an ultrathin LiF layer on Al electrodes used in molecular electronics. The LiF layer creates a sharp density of states (DOS), as in a scanning-tunneling microscope (STM) tip. The sharp DOS, coupled with the DOS of the molecule leads to negative differential resistance (NDR). Electron transfer between oriented molecules occurs via resonant tunneling. The I-V characteristic for a thin-film of tris (8-hydroxyquinoline)- aluminum (AlQ) molecules, oriented using electric-field poling, and sandwiched between two Al/LiF electrodes is in excellent agreement with theory. This molecular device presents a new paradigm for a convenient, robust, inexpensive alternative to STM or mechanical break-junction structures.",0402257v1 2004-05-06,The antiferromagnetic transition of UPd2Al3 break-junctions: A new realization of N-shaped current-voltage characteristics,"We have investigated metallic break junctions of the heavy-fermion compound UPd2Al3 at low temperatures between 0.1K and 9K and in magnetic fields up to 8T. Both the current-voltage I(V) characteristics and the dV/dI (V) spectra clearly showed the superconducting ($T_{\rm c}\simeq$ 1.8K) as well as the antiferromagnetic ($T_{\rm N}\simeq$14K) transition at low temperatures when the bias voltage is raised. The junctions with lateral size of order 200nm had huge critical current densities around $5\times 10^{10} A/m^2 at the antiferromagnetic transition and hysteretic I(V) characteristics. Degrading the quality of the contacts by in situ increasing the local residual resistivity reduced the hysteresis. We show that those hysteretic I(V) curves can be reproduced theoretically by assuming the constriction to be in the thermal regime. It turns out that these point contacts represent non-linear devices with N-shaped I(V) characteristics that have a negative differential resistance like an Esaki tunnel diode.",0405118v1 2004-05-11,Weak links and phase slip centers in superconducting MgB2 wires,"MgB2 superconducting wires were produced by the Mg diffusion method. Scanning electron microscopy (SEM), optical microscopy, dispersive x-ray analysis (EDS) and XRD diffraction were used to study the physical structure and content of the wires. Magnetic properties (Tcm, Hc1, Hc2, Jc by the Bean model) were obtained with a SQUID magnetometer, and transport properties (Tcr, Hc2, resistivity and residual resistivity ratio) were measured using a standard four-lead configuration. The V-I characteristics of the wires close to the critical temperature showed a staircase response, which was attributed to the presence of weak links, creating phase slip centers. The origin of those weak links is discussed in relation to their formation and structure.",0405219v1 2004-05-27,"Magnetic, electrical resistivity, heat-capacity and thermopower anomalies in CeCuAs2","The results of magnetic susceptibility, electrical resistivity ($\rho$), heat-capacity (C) and thermopower (S) measurements on CeCuAs2, forming in ZrCuSi2-type tetragonal structure, are reported. Our investigations reveal that Ce is trivalent and there is no clear evidence for long range magnetic ordering down to 45 mK. The $\rho$ behavior is notable in the sense that (i) the temperature (T)-coefficient of $\rho$ is negative in the entire range of measurement (45 mK to 300 K) with large values of $\rho$, while S behavior is typical of metallic Kondo lattices, and (ii) $\rho$ is proportional to T-0.6 at low temperatures, without any influence on the exponent by the application of a magnetic field, which does not seem to classify this compound into hither-to-known non-Fermi liquid (NFL) systems. In contrast to the logarithmic increase known for NFL systems, C/T measured down to 0.5 K exhibits a fall below 2 K. The observed properties of this compound are unusual among Ce systems.",0405638v1 2004-06-24,"On Electron Transport in ZrB12, ZrB2 and MgB2","We report on measurements of the temperature dependence of resistivity, $\rho(T)$, for single crystal samples of ZrB$_{12}$, ZrB$_{2}$ and polycrystalline samples of MgB$_{2}$. It is shown that cluster compound ZrB$_{12}$ behaves like a simple metal in the normal state, with a typical Bloch -- Gr\""uneisen $\rho(T)$ dependence. However, the resistive Debye temperature, $T_{R}=300 K$, is three times smaller than $T_{D}$ obtained from specific heat data. We observe the $T^{2}$ term in $\rho(T)$ of these borides, which could be interpreted as an indication of strong electron-electron interaction. Although the $\rho (T)$ dependence of ZrB$_{12}$ reveals a sharp superconductive transition at $T_{c}=6.0 K$, no superconductivity was observed for single crystal samples of ZrB$_{2}$ down to $1.3 K$.",0406615v1 2004-07-07,Kondo Behavior of U in CaB$_6$,"Replacing U for Ca in semiconducting CaB$_6$ at the few at.% level induces metallic behaviour and Kondo-type phenomena at low temperatures, a rather unusual feature for U impurities in metallic hosts. For Ca$_{0.992}$U$_{0.008}$B$_6$, the resistance minimum occurs at $T$ = 17 K. The subsequent characteristic logarithmic increase of the resistivity with decreasing temperature merges into the expected $T^2$ dependence below 0.8 K. Data of the low-temperature specific heat and the magnetization are analyzed by employing a simple resonance-level model. Analogous measurements on LaB$_6$ with a small amount of U revealed no traces of Kondo behavior, above 0.4 K.",0407158v1 2004-08-11,"Conductivity, weak ferromagnetism and charge instability in $α-MnS$ single crystal","The temperature dependence of resistivity, magnetization and electron-spin resonance of the $\alpha- MnS $ single crystal were measured in temperature range of $5 K < T < 550 K$. Magnetization hysteresis in applied magnetic field up to 0.7 T at $T=5 K, 77 K, 300 K$, irreversible temperature behavior of magnetization and resistivity were found . The obtained data were explained in terms of degenerate tight binding model using random phase approximation. The contribution of holes in $t_{2g}$ and $e_g$ bands of manganese ions to the conductivity, optical absorbtion spectra and charge instability in $\alpha -MnS $ were studied. Charge susceptibility maxima resulted from the competition of the on-site Coulomb interaction between the holes in different orbitals and small hybridization of sub-bands were calculated at $T=160 K, 250 K, 475 K$.",0408232v1 2004-08-26,Deviations from plastic barriers in Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ thin films,"Resistive transitions of an epitaxial Bi$_2$Sr$_2$CaCu$_2$O$_{8+\delta}$ thin film were measured in various magnetic fields ($H\parallel c$), ranging from 0 to 22.0 T. Rounded curvatures of low resistivity tails are observed in Arrhenius plot and considered to relate to deviations from plastic barriers. In order to characterize these deviations, an empirical barrier form is developed, which is found to be in good agreement with experimental data and coincide with the plastic barrier form in a limited magnetic field range. Using the plastic barrier predictions and the empirical barrier form, we successfully explain the observed deviations.",0408555v2 2004-08-27,Examination of the c-axis resistivity of Bi_{2}Sr_{2-x}La_xCuO_{6+δ} in magnetic fields up to 58 T,"We measure the magnetic-field dependence of the c-axis resistivity, \rho_c(H), in a series of Bi_{2}Sr_{2-x}La_xCuO_{6+\delta} (BSLCO) single crystals for a wide range of doping using pulsed magnetic fields up to 58 T. The behavior of \rho_c(H) is examined in light of the recent determination of the upper critical field H_{c2} for this material using Nernst effect measurements. We find that the peak in \rho_c(H) shows up at a field H_p that is much lower than H_{c2} and there is no discernable feature in \rho_c(H) at H_{c2}. Intriguingly, H_p shows a doping dependence similar to that of T_c, and there is an approximate relation k_{B}T_c \simeq {1/2}g\mu_{B}H_p. Moreover, we show that the data for the lowest-T_c sample can be used to estimate the pseudogap closing field H_{pg}, but the method to estimate H_{pg} proposed by Shibauchi {\it et al.} [Phys. Rev. Lett. {\bf 86}, 5763 (2001)] must be modified to apply to the BSLCO system.",0408603v1 2004-10-06,Ballistic resistivity in aluminum nanocontacts,"One of the major industrial challenges is to profit from some fascinating physical features present at the nanoscale. The production of dissipationless nanoswitches (or nanocontacts) is one of such attractive applications. Nevertheless, the lack of knowledge of the real efficiency of electronic ballistic/non dissipative transport limits future innovations. For multi-valent metallic nanosystems -where several transport channels per atom are involved- the only experimental technique available for statistical transport characterization is the conductance histogram. Unfortunately its interpretation is difficult because transport and mechanical properties are intrinsically interlaced. We perform a representative series of semiclassical molecular dynamics simulations of aluminum nanocontact breakages, coupled to full quantum conductance calculations, and put in evidence a linear relationship between the conductance and the contact minimum cross-section for the geometrically favored aluminum nanocontact configurations. Valid in a broad range of conductance values, such relation allows the definition of a transport parameter for nanomaterials, that represents the novel concept of ballistic resistivity.",0410138v1 2004-12-01,Magnetoresistive Effects in Ferromagnet-Superconductor Multilayers,"We consider a nanoscale system consisting of Manganite-ferromagnet and Cuprate-superconductor multilayers in a spin valve configuration. The magnetization of the bottom Manganite-ferromagnet is pinned by a Manganite-antiferromagnet. The magnetization of the top Manganite-ferromagnet is coupled to the bottom one via indirect exchange through the superconducting layers. We study the behavior of the critical temperature and the magnetoresistance as a function of an externally applied parallel magnetic field, when the number of Cuprate-superconductor layers are changed. There are two typical behaviors in the case of a few monolayers of the Cuprates: a) For small magnetic fields, the critical temperature and the magnetoresistance change abruptly when the flipping field of the top Manganite-ferromagnet is reached. b) For large magnetic fields, the multilayered system re-enters the zero-resistance (superconducting) state after having become resistive (normal).",0412005v1 2004-12-12,Effect of oxygen content on the transport properties and magnetoresistance in [Ca$_{2}$CoO$_{3-δ}$]$_{0.62}$[CoO$_{2}$] single crystals,"Transport property is investigated in [Ca$_{2}$CoO$_{3-\delta}$]$_{0.62}$[CoO$_{2}$] single crystals obtained by varying annealing conditions. The $\rho_{ab}(T)$ exhibits a resistivity minimum, and the temperature corresponding to this minimum increases with the loss of oxygen content, indicative of the enhancement of spin density wave (SDW). Large negative magnetoresistance (MR) was observed in all single crystals [Ca$_{2}$CoO$_{3-\delta}$]$_{0.62}$[CoO$_{2}$], while a magnetic-field-driven insulator-to-metal (IM) transition in oxygen annealed samples. These results suggest a ferromagnetic correlation in system enhanced by oxygen content. In addition, a low temperature thermal activation resistivity induced by fields was observed in single crystals annealed in oxygen atmosphere.",0412298v1 2004-12-27,Ferromagnetism and possible heavy fermion behavior in single crystals of NdOs$_4$Sb$_{12}$,"Single crystals of the filled-skutterudite compound NdOs$_4$Sb$_{12}$ have been investigated by means of electrical resistivity, magnetization, and specific heat measurements. The NdOs$_4$Sb$_{12}$ crystals have the LaFe$_4$P$_{12}$-type cubic structure with a lattice parameter of 9.3 \AA. Possible heavy-fermion behavior is inferred from specific heat measurements, which reveal a large electronic specific heat coefficient $\gamma \approx 520$ mJ/mol-K$^2$, corresponding to an effective mass $m^* \sim$ 98 $m_e$. Features related to a ferromagnetic transition at {$\sim$ 0.9 K} can be observed in electrical resistivity, magnetization and specific heat. Conventional Arrott-plot analysis indicates that NdOs$_4$Sb$_{12}$ conforms to mean-field ferromagnetism.",0412713v3 2005-02-03,"Transverse ""resistance overshoot"" in a Si/SiGe two-dimensional electron gas in the quantum Hall effect regime","We investigate the peculiarities of the ""overshoot"" phenomena in the transverse Hall resistance R_{xy} in Si/SiGe. Near the low magnetic field end of the quantum Hall effect plateaus, when the filling factor \nu approaches an integer i, R_{xy} overshoots the normal plateau value h/ie^2. However, if magnetic field B increases further, R_{xy} decreases to its normal value. It is shown that in the investigated sample n-Si/Si_{0.7}Ge_{0.3}, overshoots exist for almost all \nu. Existence of overshoot in R_{xy} observed in different materials and for different \nu, where splitting of the adjacent Landau bands has different character, hints at the common origin of this effect. Comparison of the experimental curves R_{xy}(\nu) for \nu = 3 and \nu = 5 with and without overshoot showed that this effect exist in the whole interval between plateaus, not only in the region where R_{xy} exceeds the normal plateau value.",0502094v1 2005-03-03,Transport properties of diluted magnetic semiconductors: Dynamical mean field theory and Boltzmann theory,"The transport properties of diluted magnetic semiconductors (DMS) are calculated using dynamical mean field theory (DMFT) and Boltzmann transport theory. Within DMFT we study the density of states and the dc-resistivity, which are strongly parameter dependent such as temperature, doping, density of the carriers, and the strength of the carrier-local impurity spin exchange coupling. Characteristic qualitative features are found distinguishing weak, intermediate, and strong carrier-spin coupling and allowing quantitative determination of important parameters defining the underlying ferromagnetic mechanism. We find that spin-disorder scattering, formation of bound state, and the population of the minority spin band are all operational in DMFT in different parameter range. We also develop a complementary Boltzmann transport theory for scattering by screened ionized impurities. The difference in the screening properties between paramagnetic ($T>T_c$) and ferromagnetic ($T fc) by the percolation power law returns a critical exponent t value of 2.0 +/- 0.2 at room temperature and 2.6 +/-0.2 at 5 K. The increase of t is ascribed to the influence of the grain boundaries on the electrical conduction process at low temperature.",0703367v1 2007-03-25,"Origin of superconductivity in nominally ""undoped"" T'-La$_{2-x}$Y$_{x}$CuO$_{4}$ films","We have systematically studied the transport properties of the La$_{2-x}$Y$_{x}$CuO$_{4}$(LYCO) films of T'-phase ($0.05\leq x \leq 0.30$). In this nominally ""undoped"" system, superconductivity was acquired in certain Y doping range ($0.10\leq x \leq 0.20$). Measurements of resistivity, Hall coefficients in normal states and resistive critical field ($H^\rho_{c2}$)in superconducting states of the T'-LYCO films show the similar behavior as the known Ce-doped n-type cuprate superconductors, indicating the intrinsic electron-doping nature. The charge carriers are induced by oxygen deficiency. Non-superconducting Y-doped Pr- or Nd-based T'-phase cuprate films were also investigated for comparison, suggesting the crucial role of the radii of A-site cations in the origin of superconductivity in the nominally ""undoped"" cuptates. Based on a reasonable scenario in the microscopic reduction process, we put forward a self-consistent interpretation of these experimental observations.",0703643v1 2005-11-13,Non-radiating and radiating configurations driven by left-handed metamaterials,"It is shown that a pair of identical emitters (e.g. wire dipole antennas) in the focal points of a disc, made of left-handed metamaterial (a ""perfect"" lens), form a non-radiating electromagnetic configuration. The emitters are fed with voltages of equal magnitude and pi-out-of-phase. Detailed finite-difference time-domain (FDTD) modeling shows that there are non-propagating electromagnetic fields generated - fields that remain confined within the region between the emitters and the lens. The energy balance of the system shows that the radiation resistance of the system is very low. This means that the input power is converted to heat in the volume of the lens and only a small fraction of it is radiated. The system performance shows that disturbing the configuration of the non-propagating electromagnetic fields with the presence of an externally introduced object stimulates radiation. This suggests possible detector applications. In-phase feeding voltages are also studied with the consequence that the radiation resistance of the antennae is increased.",0511113v1 2007-04-16,Memory function formalism approach to electrical conductivity and optical response of dilute magnetic semiconductors,"A combination of the memory function formalism and time-dependent density-functional theory is applied to transport in dilute magnetic semiconductors. The approach considers spin and charge disorder and electron-electron interaction on an equal footing. Within the weak disorder limit and using a simple parabolic approximation for the valence band we show that Coulomb and exchange scattering contributions to the resistivity in GaMnAs are of the same order of magnitude. The positional correlations of defects result in a significant increase of Coulomb scattering, while the suppression of localized spin fluctuations in the ferromagnetic phase contributes substantially to the experimentally observed drop of resistivity below T_c. A proper treatment of dynamical screening and collective excitations is essential for an accurate description of infrared absorption.",0704.2061v1 2007-05-15,"Magnetic, magneto-thermal and magneto-transport properties in SmMn2Si2-xGex compounds","The effect of Ge substitution for Si in SmMMn2Si2-xGex compounds has been studied. The Sm ordering temperature is found to be much larger in the compound with x=2, as compared to the compounds with x=0 and 1. The increase in the intra layer Mn-Mn distance is found to be responsible for this increase. Among these three compounds, SmMn2Ge2 is found to show re-entrant ferromagnetism at low temperatures. The magnetic contribution to the heat capacity has been found in all the three compounds. The splitting of the ground state multiplet has been estimated by fitting the magnetic part of the heat capacity data using the Schottky formula. The isothermal magnetic entropy change is found to remain the same for x=0 and 1, but decrease in the compound with x=2, though the nature of magnetic transition changes from second order to first order, as x is increased from 0 to 2. The electrical resistivity increases with Ge concentration. The excess resistivity in the antiferromagnetic region has been calculated.",0705.2237v1 2007-06-01,Anomalous magnetoresistance of EuB$_{5.99}$C$_{0.01}$: Enhancement of magnetoresistance in systems with magnetic polarons,"We present results of measurements of electrical, magnetic and thermal properties of EuB$_{5.99}$C$_{0.01}$. The observed anomalously large negative magnetoresistance as above, so below the Curie temperature of ferromagnetic ordering $T_C$ is attributed to fluctuations in carbon concentration. Below $T_C$ the carbon richer regions give rise to helimagnetic domains, which are responsible for an additional scattering term in the resistivity, which can be suppressed by a magnetic field. Above $T_C$ these regions prevent the process of percolation of magnetic polarons (MPs), acting as ""spacers"" between MPs. We propose that such ""spacers"", being in fact volumes incompatible with existence of MPs, may be responsible for the decrease of the percolation temperature and for the additional (magneto)resistivity increase in systems with MPs.",0706.0091v1 2007-07-03,Spatial correlation of linear and nonlinear electron transport in superconducting microwave resonator: laser scanning microscopy analysis,"Spatially-resolved techniques of laser scanning microscopy (LSM) have been used to image simultaneously the spatial variations of (i) rf current flow, J$_RF$(x,y), of (ii) areas of resistive dissipation and (iii) the sources of microwave nonlinearity (NL) in an operating superconducting resonator. The RF power dependent spatial evolution of these linear and NL microwave properties in the meander strip YBCO/LAO superconducting resonator have been LSM probed at different temperatures below Tc. The influence of both topologies of the twin-domain YBCO structure and of J$_RF$(x,y) peaks at the edges of superconducting strip line on its NL properties was analyzed in detail with a micron-scale spatial resolution. Result shows the resistive origin of the dominant sources of microwave NLs",0707.0358v1 2007-07-04,Resistive Switching in Cr doped SrTiO3: An X-ray Absorption Spectroscopy study,"X-ray absorption spectroscopy was used to study the microscopic origin of conductance and resistive switching in chromium doped strontium titanate (Cr:SrTiO3). Differences in the x-ray absorption near edge spectroscopy (XANES) at the Cr K-edge indicate that the valence of Cr changes from 3+ to 4+ underneath the anode of our sample device after the application of an electric field. Spatially resolved x-ray fluorescence microscopy ($\mu$-XRF) maps show that the Cr4+ region retracts from the anode-Cr:SrTiO3 interface after a conducting state has been achieved. This interface region is studied with extended x-ray absorption fine structure (EXAFS) and the results are compared with structural parameters obtained from density functional theory (DFT) calculations. They confirm that oxygen vacancies which are localized at the octahedron with a Cr at its center are introduced at the interface. It is proposed that the switching state is not due to a valence change of chromium but caused by changes of oxygen vacancies at the interface.",0707.0655v1 2007-08-21,"Negative differential resistance of Styrene on an ideal Si[111] surface: dependence of the I-V characteristics on geometry, surface doping and shape of the STM-tip","We study the electron transport properties through a supported organic molecule styrene (C8H8) on an ideal silicon surface Si[111] and probed by a STM-tip. The I-V characteristics and the differential conductance of the molecule are calculated using a self consistent approach based on non equilibrium Green's functions. Two different adsorption configurations for the molecule on the surface were considered which corresponds to a global and a local minimum of the total energy. In both cases we find a negative differential resistance (NDR) in a given interval of bias voltages. This effect is controlled by the states available close to the Fermi level of the surface and can be manipulated by properly doping the substrate. We also analyze the influence of the tip-shape on the I-V characteristics.",0708.2834v1 2007-12-21,Vibronic polarons: comments on a model for the colossal field-resistance effects in manganites,"In addition to mechanisms already proposed to account for the formation in manganites of a small-polaron superlattice above the Curie temperature Tc and to a metallic-like sea of large polarons below Tc, we now consider other observed colossal-resistance inducing fields, such as magnetic, electric, photon, or strain fields. We attribute the charge-ordered phase formation to the occurrence of strong dipolar binding of vibronic small polarons arising from the phonon coupling of highly polarizable two-level orbital systems. These species having associated inherent electric and magnetic off-center dipoles, they couple to the external fields leading to the observed colossal effects. The random phase appears due to polaron band widening in the external field.",0712.3803v1 2008-03-05,"The behavior of magnetic ordering and the KOndo effect in the alloys, Ce2Rh(1-x)Co(x)Si3: Evidence from bulk studies for Fermi-surface change during magnetic ordering - QCP transformation and applicability of SDW pictur","The results of magnetic susceptibility, electrical resistivity (rho), and heat capacity measurements as a function of temperature are reported for the alloys, Ce2Rh(1-x)Co(x)Si3, crystallizing in an AlB2-derived hexagonal strcture. Ce2RhSi3 exhibits antiferromagnetic ordering at 7 K. The Neel temperature decreases gradually with the increase in Co concentration. For x greater than 0.6, no magnetic ordering is observed down to 0.5 K. Interestingly, the x= 0.6 alloy exhibits signatutes of non-Fermi liquid behavior, while the Co end member is a Fermi liquid. Thus, a transformation of magnetic ordering state to non-magnetism via non-Fermiliquid state by isoelectronic chemical doping is evident in this solid solution. The electrical resistivity data for x= 0.2 and 0.3 alloys show an upturn at respective Neel temperatures, establishing the formation of a magnetism-induced pseudo-gap for these intermediate compositions alone as though there is a gradual Fermi surface transformation as the quantum critical point is approached.",0803.0652v1 2008-03-09,"Upper critical field, Hall effect and magnetoresistance in the iron-based layered superconductor LaFeAsO_{0.9}F_{0.1-δ}","By using a two-step method, we successfully synthesized the iron based new superconductor LaFeAsO_{0.9}F_{0.1-\delta}$. The resistive transition curves under different magnetic fields were measured, leading to the determination of the upper critical field Hc2(T) of this new superconductor. The value of Hc2 at zero temperature is estimated to be about 50 Tesla roughly. In addition, the Hall effect and magnetoresistance were measured in wide temperature region. A negative Hall coefficient R_H has been found, implying a dominant conduction mainly by electron-like charge carriers in this material. The charge carrier density determined at 100 K is about 9.8E20cm^{-3}, which is close to the cuprate superconductors. It is further found that the magnetoresistance does not follow Kohler's law. Meanwhile, the different temperature dependence behaviors of resistivity, Hall coefficient, and magnetoresistance have anomalous properties at about 230 K, which may be induced by some exotic scattering mechanism.",0803.1288v2 2008-03-12,Electron transport and thermoelectric properties of layered perovskite LaBaCo2O5.5,"We have investigated the systematic transport properties of the layered 112-type cobaltite LaBaCo2O5.5 by means of electrical resistivity, magnetoresistance, electroresistance and thermoelectric measurements in various conditions. In order to understand the complex conduction mechanism of LaBaCo2O5.5, the transport data have been analyzed using different theoretical models. The system shows semiconductor-semiconductor like transition (TSC) around 326K, corresponding to ferromagnetic transition and in the low temperature region resistivity data follows the Motts variable range hopping model. Interestingly, near and below the room temperature this compound depicts significant change in electro- and magnetoresistance behavior, the latter one is noteworthy near the magnetic phase boundary. The temperature dependence of thermopower, S(T), exhibits p-type polaronic conductivity in the temperature range of 60-320K and reaches a maximum value of 303 uV/K (at 120K). In the low temperature AFM region, the unusual S(T) behavior, generally observed for the cobaltite series LnBaCo2O5.5 (Ln = Rare Earth), is explained by the electron magnon scattering mechanism as previously described for perovskite manganites.",0803.1806v1 2008-03-14,From Ohmic to Ballistic Transport in Oriented Graphite,"In this work we show that for a quasi-2D system of size $\Omega$ and thickness $t$ the resistance goes as $(2\rho/\pi t)\ln(\Omega/W)$, diverging logarithmically with the size. Measurements in highly oriented pyrolytic graphite (HOPG) as well as numerical simulations confirm this relation. Furthermore, we present an experimental method that allows us to obtain the carriers mean free path $l(T)$, the Fermi wavelength $\lambda(T)$ and the mobility $\mu(T)$ directly from experiments without adjustable parameters. Measuring the electrical resistance through microfabricated constrictions in HOPG and observing the transition from ohmic to ballistic regime we obtain that $0.2 \mu$m $\lesssim l \lesssim 10 \mu$m, $0.1 \mu$m $\lesssim \lambda \lesssim 2 \mu$m and a mobility $5 \times 10^4$ cm$^2$/Vs $ \lesssim \mu \lesssim 4 \times 10^7$ cm$^2$/Vs when the temperature decreases from 270K to 3K. A comparison of these results with those from literature indicates that conventional, multiband Boltzmann-Drude approaches are inadequate for oriented graphite. The upper value obtained for the mobility is much larger than the mobility graphene samples of micrometer size can have.",0803.2203v2 2008-03-19,Theory of quantum metal to superconductor transitions in highly conducting systems,"We derive the theory of the quantum (zero temperature) superconductor to metal transition in disordered materials when the resistance of the normal metal near criticality is small compared to the quantum of resistivity. This can occur most readily in situations in which ``Anderson's theorem'' does not apply. We explicitly study the transition in superconductor-metal composites, in an s-wave superconducting film in the presence of a magnetic field, and in a low temperature disordered d-wave superconductor. Near the point of the transition, the distribution of the superconducting order parameter is highly inhomogeneous. To describe this situation we employ a procedure which is similar to that introduced by Mott for description of the temperature dependence of the variable range hopping conduction. As the system approaches the point of the transition from the metal to the superconductor, the conductivity of the system diverges, and the Wiedemann-Franz law is violated. In the case of d-wave (or other exotic) superconductors we predict the existence of (at least) two sequential transitions as a function of increasing disorder: a d-wave to s-wave, and then an s-wave to metal transition.",0803.2902v2 2008-03-23,Origin of negative differential resistance in a strongly coupled single molecule-metal junction device,"A new mechanism is proposed to explain the origin of negative differential resistance (NDR) in a strongly coupled single molecule-metal junction. A first-principles quantum transport calculation in a Fe-terpyridine linker molecule sandwiched between a pair of gold electrodes is presented. Upon increasing applied bias, it is found that a new phase in the broken symmetry wavefunction of the molecule emerges from the mixing of occupied and unoccupied molecular orbital. As a consequence, a non-linear change in the coupling between molecule and lead is evolved resulting to NDR. This model can be used to explain NDR in other class of metal-molecule junction device.",0803.3342v1 2008-04-13,Conductance of p-n-p graphene structures with 'air-bridge' top gates,"We have fabricated graphene devices with a top gate separated from the graphene layer by an air gap--a design which does not decrease the mobility of charge carriers under the gate. This gate is used to realise p-n-p structures where the conducting properties of chiral carriers are studied. The band profile of the structures is calculated taking into account the specifics of the graphene density of states and is used to find the resistance of the p-n junctions expected for chiral carriers. We show that ballistic p-n junctions have larger resistance than diffusive ones. This is caused by suppressed transmission of chiral carriers at angles away from the normal to the junction.",0804.2081v3 2008-06-16,"Metal-insulator transition and giant anisotropic magnetoresistance in ultra thin (Ga,Mn)As","MBE-grown, 5 nm-thick annealed Ga0.95Mn0.05As films with Tc~90K demonstrate transition from metallic to insulating state below To~10K, where sheet resistances Rsh~h/e2 and both longitudinal Rxx and transverse Rxy components become comparable. Below metal-insulator transition we found giant anisotropic magnetoresistance (GAMR), which depends on orientation of magnetization to crystallographic axes and manifests itself in positive magnetoresistance near 50% for Rxx at T=1.7K, H//[110] crystallographic direction and parallel to current in contrast to smaller and negative magnetoresistance for H// direction. We connect GAMR with anisotropic spin-orbit interaction resulting in formation of high- and low- resistance states with different localization along non-equivalent easy axes.",0806.2590v1 2008-06-28,Theory of spin magnetohydrodynamics,"We develop a phenomenological hydrodynamic theory of coherent magnetic precession coupled to electric currents. Exchange interaction between electron spin and collective magnetic texture produces two reciprocal effects: spin-transfer torque on the magnetic order parameter and the Berry-phase gauge field experienced by the itinerant electrons. The dissipative processes are governed by three coefficients: the ohmic resistance, Gilbert damping of the magnetization, and the ""beta coefficient"" describing viscous coupling between magnetic dynamics and electric current, which stems from spin mistracking of the magnetic order. We develop general magnetohydrodynamic equations and discuss the net dissipation produced by the coupled dynamics. The latter in particular allows us to determine a lower bound on the magnetic-texture resistivity.",0806.4656v2 2008-07-28,Transport anomalies across the quantum limit in semimetallic Bi$_{0.96}$Sb$_{0.04}$,"We report on a study of electronic transport in semi-metallic Bi$_{0.96}$Sb$_{0.04}$. At zero field, the system is a very dilute Fermi liquid displaying a T$^{2}$ resistivity with an enhanced prefactor. Quantum oscillations in resistivity as well as in Hall, Nernst and Seebeck responses of the system are detectable and their period quantifies the shrinking of the Fermi surface with antimony doping. For a field along the trigonal axis, the quantum limit was found to occur at a field as low as 3T. An ultraquantum anomaly at twice this field was detected in both charge transport and Nernst response. Its origin appears to lie beyond the one-particle picture and linked to unidentified many-body effects.",0807.4432v1 2008-07-30,Ultra-Thin Silver Films obtained by Sequential Quench-Anneal Processing,"We have used the two-step growth technique, quench condensing followed by an anneal, to grow ultra thin films of silver on glass substrates. As has been seen with semiconductor substrates this process produces a metastable homogeneous covering of silver. By measuring the in situ resistance of the film during growth we are able to see that the low temperature growth onto substrates held at 100 Kelvin produces a precursor phase that is insulating until the film has been annealed. The transformation of the precursor phase into the final, metallic silver film occurs at a characteristic temperature near 150K where the sample reconstructs. This reconstruction is accompanied by a decrease in resistance of up to 10 orders of magnitude.",0807.4948v1 2008-08-09,Electronic transport and specific heat of 1T- VSe2,"The results of low temperature thermoelectric power and the specific heat of 1T-VSe2 (Vanadium diselenide) have been reported along with the electrical resistivity, and Hall coefficient of the compound. The Charge Density Wave (CDW) transition is observed near 110K temperature in all these properties. The Thermoelectric power has been measured from 15K to 300K spanning the incommensurate and commensurate CDW regions. We observed a weak anomaly at the CDW transition for the first time in the specific heat of VSe2. The linear temperature dependence of resistivity and thermoelectric power at higher temperatures suggests a normal metallic behavior and electron-phonon scattering above the CDW transition. The positive thermoelectric power and negative Hall coefficient along with strongly temperature dependent behavior in the CDW phase suggest a mixed conduction related to the strongly hybridized s-p-d bands in this compound.",0808.1332v2 2008-08-11,Non-trivial length dependence of the conductance and negative differential resistance in atomic molecular wires,"We study the electronic and transport properties of two novel molecular wires made of atomic chains of carbon atoms (polyynes) capped with either, benzene-thiols or pyridines. While both molecules are structurally similar, the electrical conductance of benzene-thiol-capped chains attached to gold electrodes is found to be much higher than that of pyridine-capped chains. We predict that the conductance is almost independent of molecular length, which suggests that these molecules could be ideal molecular wires for sub-10 nm circuitry. Both systems exhibit negative differential resistance (NDR) but its origin and characteristics depend on the type of molecule. We find a novel type of NDR mechanism produced by the movement of the LUMO resonance with bias. We also show that by gating the pyridine-capped molecules it is possible to make the NDR disappear and dramatically modify the $I$-$V$ characteristics and the length dependence.",0808.1494v2 2008-08-21,Electrons and holes in Si quantum well: a room-temperature transport and drag resistance study,"We investigate carrier transport in a single 22 nm-thick double-gated Si quantum well device, which has independent contacts to electrons and holes. Conductance, Hall density and Hall mobility are mapped in a broad double-gate voltage window. When the gate voltage asymmetry is not too large only either electrons or holes occupy the Si well and the Hall mobility shows the fingerprints of volume inversion/accumulation. At strongly asymmetric double-gate voltage an electric field induced electron-hole (EH) bi-layer is formed inside the well. The EH drag resistance R_{he} is explored at balanced carrier densities: R_{he} decreases monotonically from 860 to 37 Ohms when the electron and hole density is varied between ~0.4-1.7x10^{16} m^{-2}.",0808.2914v1 2008-10-27,Abrupt Emergence of Pressure-Induced Superconductivity of 34 K in SrFe2As2: A Resistivity Study under Pressure,"We report resistivity measurement under pressure in single crystals of SrFe_2As_2, which is one of the parent materials of Fe-based superconductors. The structural and antiferromagnetic (AFM) transition of T_0 = 198 K at ambient pressure is suppressed under pressure, and the ordered phase disappears above P_c ~ 3.6-3.7 GPa. Superconductivity with a sharp transition appears accompanied by the suppression of the AFM state. T_c exhibits a maximum of 34.1 K, which is realized close to the phase boundary at P_c. This T_c is the highest among those of the stoichiometric Fe-based superconductors.",0810.4856v2 2008-12-11,Difference of Oxide Hetero-Structure Junctions with Semiconductor Electronic Devices,"Charge carrier injection performed in Pr0.7Ca0.3MnO3 (PCMO) hetero-structure junctions exhibits stable without electric fields and dramatic changes in both resistances and interface barriers, which are entirely different from behaviors of semiconductor devices. Disappearance and reversion of interface barriers suggest that the adjustable resistance switching of such hetero-structure oxide devices should associate with motion of charge carriers across interfaces. The results suggested that injected carriers should be still staying in devices and resulted in changes in properties, which guided to a carrier self-trapping and releasing picture in strongly correlated electronic framework. Observations in PCMO and oxygen deficient CeO2 devices show that oxides as functional materials could be used in microelectronics with some novel properties, in which interface is very important.",0812.2071v1 2008-12-11,Evidence for Coexistence of Superconductivity and Magnetism in Single Crystals of Co-doped SrFe$_2$As$_2$,"In order to investigate whether magnetism and superconductivity coexist in Co-doped SrFe$_2$As$_2$, we have prepared single crystals of SrFe$_{2-x}$Co$_x$As$_2$, $x$ = 0 and 0.4, and characterized them via X-ray diffraction, electrical resistivity in zero and applied field up to 9 T as well as at ambient and applied pressure up to 1.6 GPa, and magnetic susceptibility. At $x$ = 0.4, there is both magnetic and resistive evidence for a spin density wave transition at 120 K, while $T_c$ = 19.5 K - indicating coexistent magnetism and superconductivity. A discussion of how these results compare with reported results, both in SrFe$_{2-x}$Co$_x$As$_2$ and in other doped 122 compounds, is given.",0812.2091v1 2009-01-10,"Wafer-Scale, Sub-5 nm Junction Formation by Monolayer Doping and Conventional Spike Annealing","We report the formation of sub-5 nm ultrashallow junctions in 4 inch Si wafers enabled by the molecular monolayer doping of phosphorous and boron atoms and the use of conventional spike annealing. The junctions are characterized by secondary ion mass spectrometry and non-contact sheet resistance measurements. It is found that the majority (~70%) of the incorporated dopants are electrically active, therefore, enabling a low sheet resistance for a given dopant areal dose. The wafer-scale uniformity is investigated and found to be limited by the temperature homogeneity of the spike anneal tool used in the experiments. Notably, minimal junction leakage currents (<1 uA/cm2) are observed which highlights the quality of the junctions formed by this process. The results clearly demonstrate the versatility and potency of the monolayer doping approach for enabling controlled, molecular-scale ultrashallow junction formation without introducing defects in the semiconductor.",0901.1396v1 2009-02-10,Spontaneous and low-field magnetoimpedance in La0.7Sr0.3CoO3 and La1-xSrxMnO3 (x = 0.18-0.5),"We report ac electrical transport in La0.7Sr0.3CoO3 and La1-xSrxMnO3 (x = 0.18- 0.5) as a function of temperature and frequency in H = 0 and 60 mT. Both resistive (R) and reactive (X) components of impedance (Z = R+jX) were measured. It is shown that a smooth decrease of the resistance around the Curie temperautre in La0.7Sr0.3CoO3 transforms into an abrupt increase followed closely by a peak in R with increasing frequency. Similar behavior in R was also found in metallic compositions of the La-Sr-MnO3 series. The observed anomaly at TC is suppressed by a small dc magnetic field of H = 60 mT which rrsults in a huge ac magnetoreistance (= 30 % in manganite and =7 % in cobaltite at f = 2 MHz). The anomaly in R in zero field is also accompanied by a sudden incrases of X. While the ac magnetoresitance is negative as a function of field from 100 Hz to 30 MHz, we show that the sign of X changes and a new double peak structure develops in X for frequencies above 15 MHz.",0902.1780v1 2009-04-24,Evolution of orbital phases with particle size in nanoscale stoichiometric LaMnO3,"The thermodynamically stable long-range orbital order in bulk LaMnO3 becomes metastable at nanoscale around a critical particle size d_C~20 nm. The orbital order-disorder transition switches from reversible to irreversible at d_C while the resistance in the orbital ordered state decays by 2-4% over a time scale of ~3000s. At well below d_C, of course, a stable orbital disordered phase emerges. The orthorhombic distortion of the underlying crystallographic structure (space group Pbnm) decreases systematically with the decrease in particle size and at far below d_C (e.g., at ~10 nm), the structure becomes cubic (space group Pm-3m). Using the crystallographic and electrical resistance data, a phase diagram has been constructed showing the evolution of different orbital phases as a function of particle size across ~10 nm to bulk for stoichiometric LaMnO3.",0904.3878v3 2009-06-04,Sensitivity of Ag/Al Interface Specific Resistances to Interfacial Intermixing,"We have measured an Ag/Al interface specific resistance, 2AR(Ag/Al)(111) = 1.4 fOhm-m^2, that is twice that predicted for a perfect interface, 50% larger than for a 2 ML 50%-50% alloy, and even larger than our newly predicted 1.3 fOhmm^2 for a 4 ML 50%-50% alloy. Such a large value of 2ARAg/Al(111) confirms a predicted sensitivity to interfacial disorder and suggests an interface greater than or equal to 4 ML thick. From our calculations, a predicted anisotropy ratio, 2AR(Ag/Al)(001)/2AR(Ag/Al)(111), of more then 4 for a perfect interface, should be reduced to less than 2 for a 4 ML interface, making it harder to detect any such anisotropy.",0906.0934v1 2009-06-04,Perpendicular-current Studies of Electron Transport Across Metal/Metal Interfaces,"We review what we have learned about the scattering of electrons by the interfaces between two different metals (M1/M2) in the current-perpendicular-to-plane (CPP) geometry. In this geometry, the intrinsic quantity is the specific resistance, AR, the product of the area through which the CPP current flows times the CPP resistance. We describe results for both non-magnetic/non-magnetic (N1/N2) and ferromagnetic/non-magnetic (F/N) pairs. We focus especially upon cases where M1/M2 are lattice matched (i.e., have the same crystal structure and the same lattice parameters to within ~ 1%), because in these cases no-free-parameter calculations of 2AR agree surprisingly well with measured values. But we also list and briefly discuss cases where M1/M2 are not lattice matched, either having different crystal structures, or lattice parameters that differ by several percent. The published calculations of 2AR in these latter cases do not agree so well with measured values.",0906.0936v1 2009-06-26,Upper bound for the conductivity of nanotube networks,"Films composed of nanotube networks have their conductivities regulated by the junction resistances formed between tubes. Conductivity values are enhanced by lower junction resistances but should reach a maximum that is limited by the network morphology. By considering ideal ballistic-like contacts between nanotubes we use the Kubo formalism to calculate the upper bound for the conductivity of such films and show how it depends on the nanotube concentration as well as on their aspect ratio. Highest measured conductivities reported so far are approaching this limiting value, suggesting that further progress lies with nanowires other than nanotubes.",0906.4906v2 2009-06-29,Upper critical fields of the 11-system iron-chalcogenide superconductor FeSe$_{0.25}$Te$_{0.75}$,"We have performed electrical resistivity measurements of a polycrystalline sample of FeSe$_{0.25}$Te$_{0.75}$, which exhibits superconductivity at $T_{\rm c} \sim 14$ K, in magnetic fields up to 55 T to determine the upper critical field $\mu_{0}H_{\rm c2}$. In this compound, very large slopes of $\mu_{0}H_{\rm c2}$ at the onset, the mid-point, the zero-resistivity temperatures on superconductivity are determined to be -13.7, -10.1, and -6.9 T/K, respectively. The observed $\mu_{0}H_{\rm c2}(T)$s of this compound are considerably smaller than those expected from the Werthamer-Helfand-Hohenberg model, manifesting the Pauli limiting behavior. These results suggest that this compound has a large Maki parameter, but it is smaller than that calculated for a weak-coupling superconductor, indicating a large superconducting gap of this compound as a strong-coupling superconductor.",0906.5248v1 2009-07-17,"Phase diagram of CeFeAs$_{1-x}$P$_{x}$O obtained from electric resistivity, magnetization, and specific heat measurements","We performed a systematic study on the properties of CeFeAs$_{1-x}$P$_{x}$O ($0\leq x\leq 1$) by electrical resistivity, magnetization and specific heat measurements. The c-axis lattice constant decreases significantly with increasing P content, suggesting a remarkable chemical pressure. The Fe-3d electrons show the enhanced metallic behavior upon P-doping and undergo a magnetic quantum phase transition around $x \approx 0.4$. Meanwhile, the Ce-4f electrons develop a ferromagnetic order near the same doping level. The ferromagnetic order is vanishingly small around $x=0.9$. The data suggest a heavy-fermion-like behavior as $x\geq 0.95$. No superconductivity is observed down to 2 K. Our results show the ferromagnetic ordered state as an intermediate phase intruding between the antiferromagnetic bad metal and the nonmagnetic heavy fermion metal and support the cerium-containing iron pnictides as a unique layered Kondo lattice system.",0907.2961v2 2009-07-31,Top and side gated epitaxial graphene field effect transistors,"Three types of first generation epitaxial graphene field effect transistors (FET) are presented and their relative merits are discussed. Graphene is epitaxially grown on both the carbon and silicon faces of hexagonal silicon carbide and patterned with electron beam lithography. The channels have a Hall bar geometry to facilitate magnetoresistance measurements. FETs patterned on the Si-face exhibit off-to-on channel resistance ratios that exceed 30. C-face FETs have lower off-to-on resistance ratios, but their mobilities (up to 5000 cm2/Vs) are much larger than that for Si-face transistors. Initial investigations into all-graphene side gate FET structures are promising.",0908.0017v1 2009-08-02,Spin-dependent transport in nanocomposite C:Co films,"The magneto-transport properties of nanocomposite C:Co (15 and 40 at.% Co) thin films are investigated. The films were grown by ion beam co-sputtering on thermally oxidized silicon substrates in the temperature range from 200 to 500 degC. Two major effects are reported: (i) a large anomalous Hall effect amounting to 2 \mu ohm cm, and (ii) a negative magnetoresistance. Both the field-dependent resistivity and Hall resistivity curves coincide with the rescaled magnetization curves, a finding that is consistent with spin-dependent transport. These findings suggest that C:Co nanocomposites are promising candidates for carbon-based Hall sensors and spintronic devices.",0908.0127v1 2009-09-16,"Superconductivity at 39 K in New Iron Pnictide Oxide (Fe2As2)(Sr4(Mg,Ti)2O6)","We have discovered a new iron pnictide oxide superconductor (Fe2As2)(Sr4(Mg,Ti)2O6). This material is isostructual with (Fe2As2)(Sr4M2O6) (M = Sc, Cr), which was found in our previous study. The structure of this compound is tetragonal with a space group of P4/nmm and consists of the anti-fluorite type FeAs and perovskite-type blocking layers. The lattice constants are a = 3.935 A and c = 15.952 A for (Fe2As2)(Sr4MgTiO6). In both magnetization and resistivity measurements, this compound exhibits superconductivity below 10 K. Moreover, ratio of Mg and Ti in this compound can be changed toward Ti-rich composition. (Fe2As2)(Sr4Mg1-xTi1+xO6) phase is obtained at 0 < x as a main phase, and Tc and superconducting volume fraction increase with increasing x. The highest Tc(onset) was confirmed at 39 K for x = 0.6 in resistivity measurement.",0909.2945v3 2009-09-25,"Electrical, magnetic, magnetodielectric and magnetoabsorption studies in multiferroic GaFeO3","We report electrical, magnetic, magnetodielectric and magnetoabsorption properties of a polycrystalline GaFeO3. The resistivity measurement shows that the sample is highly insulating below 200 K and the resistivity above 200 K obey the Arrhenius law with an activation energy of Ea = 0.67 eV. An anomaly occurs in the temperature dependence of permittivity (e) near the ferrimagnetic transition temperature (TC = 228 K) in a zero magnetic field and it is suppressed under H = 60 mT which indicates a possible magnetoelectric coupling in GaFeO3 with a fractional change of de/e = -1.8% at 60 mT around TC. The coercivity (HC) of the sample increases dramatically with lowering temperature below 200 K from 0.1 T at 200 K to 0.9 T at 5 K. Magnetoabsorption was studied with a LC resonance technique and we found a close correlation between the shift in the resonance frequency due to applied magnetic field and the coercive field measured using dc magnetization measurements. Our results obtained with multiple techniques suggest that GaFeO3 is an interesting ferrimagnet with potential applications in future multiferroic devices.",0909.4609v1 2009-10-11,Anomalous Hall resistance in Ge:Mn systems with low Mn concentrations,"Taking Mn doped Germanium as an example, we evoke the consideration of a two-band-like conduction in diluted ferromagnetic semiconductor (FMS). The main argument for claiming Ge:Mn as a FMS is the occurrence of the anomalous Hall effect (AHE). Usually, the reported AHE (1) is observable at temperatures above 10 K, (2) exhibits no hysteresis, and (3) changes the sign of slope. We observed a similar Hall resistance in Mn implanted Ge with the Mn concentration as low as 0.004%. We show that the puzzling AHE features can be explained by considering a two-band-like conduction in Ge:Mn.",0910.1981v1 2009-10-20,"Sharp fall of electrical resistance for a small application of magnetic field on a metastable form of a compound, Tb5Si3, under pressure","We report an unusual sensitivity of electrical resistivity (rho) to an application of a small magnetic field in an intermetallic compound, Tb5Si3, under pressure. In this compound, there is a magnetic field-induced first-order magnetic transition at 1.8 K. Under pressure, there is a metastable magnetic phase after reducing the field to zero. This metastable phase is relatively of higher rho and interestingly a small magnetic field (less than 2 kOe) in the reverse direction results in a sharp fall of rho to restore virgin state rho. The present finding could be relevant to spintronic applications.",0910.3794v1 2009-11-11,Neutron powder diffraction investigation of the structural and magnetic properties of (La1-yYy)FeAsO,"The structural, magnetic and resistive properties of (La1-yYy)FeAsO compounds (y = 0.10, 0.20, 0.30) have been investigated by means of X-ray and neutron powder diffraction as well as by resistivity measurements. The temperatures at which the structural transition from tetragonal to orthorhombic and the magnetic ordering take place progressively reduce by similar amounts with increasing Y substitution on account of the progressive chemical pressure increase. We propose that the structural transition could be originated by a cooperative Jahn-Teller distortion involving the alignment of the fully occupied Fe 3d(z2) orbitals in the Fe plane along the y axis, leading to the branching of the cell parameters a and b. The magnetic structure develops after the occurrence of the structural transition, but before its completion.",0911.2153v1 2009-11-23,Magnetic field and contact resistance dependence of non-local charge imbalance,"Crossed Andreev reflection (CAR) in metallic nanostructures, a possible basis for solid-state electron entangler devices, is usually investigated by detecting non-local voltages in multi-terminal superconductor/normal metal devices. This task is difficult because other subgap processes may mask the effects of CAR. One of these processes is the generation of charge imbalance (CI) and the diffusion of non-equilibrium quasi-particles in the superconductor. Here we demonstrate a characteristic dependence of non-local CI on a magnetic field applied parallel to the superconducting wire, which can be understood by a generalization of the standard description of CI to non-local experiments. These results can be used to distinguish CAR and CI and to extract CI relaxation times in superconducting nanostructures. In addition, we investigate the dependence of non-local CI on the resistance of the injector and detector contacts and demonstrate a quantitative agreement with a recent theory using only material and junction characteristics extracted from separate direct measurements.",0911.4427v1 2009-12-16,Cooling dynamics and thermal interface resistance of glass-embedded metal nanoparticles,"The cooling dynamics of glass-embedded noble metal nanoparticles with diameters ranging from 4 to 26 nm were studied using ultrafast pump-probe spectroscopy. Measurements were performed probing away from the surface plasmon resonance of the nanoparticles to avoid spurious effects due to glass heating around the particle. In these conditions, the time-domain data reflect the cooling kinetics of the nanoparticle. Cooling dynamics are shown to be controlled by both thermal resistance at the nanoparticule?glass interface, and heat diffusion in the glass matrix. Moreover, the interface conductances are deduced from the experiments and found to be correlated to the acoustic impedance mismatch at the metal/glass interface.",0912.3058v1 2009-12-29,Interplay of bulk and interface effects in the electric-field driven transition in magnetite,"Contact effects in devices incorporating strongly-correlated electronic materials are comparatively unexplored. We have investigated the electrically-driven phase transition in magnetite (100) thin films by four-terminal methods. In the lateral configuration, the channel length is less than 2 $\mu$m, and voltage-probe wires $\sim$100 nm in width are directly patterned within the channel. Multilead measurements quantitatively separate the contributions of each electrode interface and the magnetite channel. We demonstrate that on the onset of the transition contact resistances at both source and drain electrodes and the resistance of magnetite channel decrease abruptly. Temperature dependent electrical measurements below the Verwey temperature indicate thermally activated transport over the charge gap. The behavior of the magnetite system at a transition point is consistent with a theoretically predicted transition mechanism of charge gap closure by electric field.",0912.5374v1 2010-01-08,Low-magnetic-field control of dielectric constant at room temperature realized in Ba0.5Sr1.5Zn2Fe12O22,"We show that room temperature resistivity of Ba0.5Sr1.5Zn2Fe12O22 single crystals increases by more than three orders of magnitude upon being subjected to optimized heat treatments. The increase in the resistivity allows the determination of magnetic field (H)-induced ferroelectric phase boundaries up to 310 K through the measurements of dielectric constant at a frequency of 10 MHz. Between 280 and 310 K, the dielectric constant curve shows a peak centered at zero magnetic field and thereafter decreases monotonically up to 0.1 T, exhibiting a magnetodielectric effect of 1.1%. This effect is ascribed to the realization of magnetic field-induced ferroelectricity at an H value of less than 0.1 T near room temperature. Comparison between electric and magnetic phase diagrams in wide temperature- and field-windows suggests that the magnetic field for inducing ferroelectricity has decreased near its helical spin ordering temperature around 315 K due to the reduction of spin anisotropy in Ba0.5Sr1.5Zn2Fe12O22.",1001.1319v1 2010-03-05,Weak superconducting fluctuations and small anisotropy of the upper critical fields in an Fe1.05Te0.85Se0.15 single crystal,"We have investigated the temperature dependence of the resistive upper critical fields ($\mu_{0}H_{\rm c2}(T)$) for an Fe$_{1.05}$Te$_{0.85}$Se$_{0.15}$ single crystal, which exhibit superconductivity at $T_{\rm c} \sim 14 K, in magnetic fields of up to 55 T. Two-dimensional feature and superconducting fluctuations of the samples are found to be weak, because the resistive broadening effect on applied magnetic fields of up to 14 T is small. The Pauli paramagnetic effect is obviously evidenced by the strong suppression of the $\mu_{0}H_{\rm c2}^{ab}(T)$ ($H \parallel ab$) curve and nearly isotropic $\mu_{0}H_{\rm c2}(0) \approx 47 T is seen for both $H \parallel ab$ and $H \parallel c$. This fact is almost identical to the results of Fe$_{1+y}$Te$_{0.6}$Se$_{0.4}$ single crystals reported previously. We have discussed that the small anisotropy of the upper critical field at low temperatures in Fe$_{1+y}$(Te,Se) systems against the variation of the Te/Se ratio.",1003.1171v3 2010-03-19,Lateral Spin Injection in Germanium Nanowires,"Electrical injection of spin-polarized electrons into a semiconductor, large spin diffusion length, and an integration friendly platform are desirable ingredients for spin-based devices. Here we demonstrate lateral spin injection and detection in germanium nanowires, by using ferromagnetic metal contacts and tunnel barriers for contact resistance engineering. Using data measured from over 80 samples, we map out the contact resistance window for which lateral spin transport is observed, manifestly showing the conductivity matching required for spin injection. Our analysis, based on the spin diffusion theory, indicates that the spin diffusion length is larger than 100 {\mu}m in germanium nanowires at 4.2 K.",1003.3787v2 2010-03-28,Scanning Gate Microscopy on Graphene: Charge Inhomogeneity and Extrinsic Doping,"We have performed scanning gate microscopy (SGM) on graphene field effect transistors (GFET), using a biased metallic nanowire coated with a dielectric layer as a contact mode tip and local top gate. Electrical transport through graphene at various back gate voltages is monitored as a function of tip voltage and tip position. Near the Dirac point, the dependence of graphene resistance on tip voltage shows a significant variation with tip position. SGM imaging reveals mesoscopic domains of electron-doped and hole-doped regions. Our measurements indicate a substantial spatial fluctuation (on the order of 10^12/cm^2) in the carrier density in graphene due to extrinsic local doping. Important sources for such doping found in our samples include metal contacts, edges of graphene, structural defects, and resist residues.",1003.5404v1 2010-04-07,Temperature dependence of the nonlocal voltage in an Fe/GaAs electrical spin injection device,"The nonlocal spin resistance is measured as a function of temperature in a Fe/GaAs spin-injection device. For nonannealed samples that show minority-spin injection, the spin resistance is observed up to room temperature and decays exponentially with temperature at a rate of 0.018\,K$^{-1}$. Post-growth annealing at 440\,K increases the spin signal at low temperatures, but the decay rate also increases to 0.030\,K$^{-1}$. From measurements of the diffusion constant and the spin lifetime in the GaAs channel, we conclude that sample annealing modifies the temperature dependence of the spin transfer efficiency at injection and detection contacts. Surprisingly, the spin transfer efficiency increases in samples that exhibit minority-spin injection.",1004.1034v1 2010-05-01,Reversible Fluorination of Graphene: towards a Two-Dimensional Wide Bandgap Semiconductor,"We report the synthesis and evidence of graphene fluoride, a two-dimensional wide bandgap semiconductor derived from graphene. Graphene fluoride exhibits hexagonal crystalline order and strongly insulating behavior with resistance exceeding 10 G$\Omega$ at room temperature. Electron transport in graphene fluoride is well described by variable-range hopping in two dimensions due to the presence of localized states in the band gap. Graphene obtained through the reduction of graphene fluoride is highly conductive, exhibiting a resistivity of less than 100 k$\Omega$ at room temperature. Our approach provides a new path to reversibly engineer the band structure and conductivity of graphene for electronic and optical applications.",1005.0113v1 2010-07-15,Quantum Hall Resistance Overshoot in 2-Dimensional Electron Gases - Theory and Experiment,"We present a systematical experimental investigation of an unusual transport phenomenon observed in two dimensional electron gases in Si/SiGe heterostructures under integer quantum Hall effect (IQHE) conditions. This phenomenon emerges under specific experimental conditions and in different material systems. It is commonly referred to as Hall resistance overshoot, however, lacks a consistent explanation so far. Based on our experimental findings we are able to develop a model that accounts for all of our observations in the framework of a screening theory for the IQHE. Within this model the origin of the overshoot is attributed to a transport regime where current is confined to co-existing evanescent incompressible strips of different filling factors.",1007.2586v1 2010-08-10,Transition from a ferromagnetic insulating to a ferromagnetic metallic state in nanoparticles of Nd0.8Sr0.2MnO3 : Study of the electronic - and magneto - transport properties,"A detailed investigation of the electronic - and magneto - transport properties of Nd0.8Sr0.2MnO3 with the variation of grain size (down to 42 nm) is presented here. Interestingly, we observe that the ferromagnetic insulating state is suppressed and a metallic state is stabilized as the grain size of the sample is reduced. As a result, metal insulator transition is observed in this low doped manganite which is insulating in nature in its bulk form. Destabilization of polaronic order in the ferromagnetic insulating state due to enhanced surface disorder on grain size reduction has been attributed to this effect. A phenomenological model has been proposed to represent the concept of destabilization of polaron formation in the surface region of the nano grains. Resistivity and magnetoresistance data have been carefully analyzed employing different suitable models. Electrical third harmonic resistance has been measured to directly probe the electrical nonlinearity in the samples.",1008.1693v1 2010-08-18,A New Strained-Silicon Channel Trench-gate Power MOSFET: Design and Analysis,"In this paper, we propose a new trench power MOSFET with strained Si channel that provides lower on resistance than the conventional trench MOSFET. Using a 20% Ge mole fraction in the Si1-xGex body with a compositionally graded Si1-xGex buffer in the drift region enables us to create strain in the channel along with graded strain in the accumulation region. As a result, the proposed structure exhibits 40% enhancement in current drivability, 28% reduction in the on-resistance and 72% improvement in peak transconductance at the cost of only 12% reduction in the breakdown voltage when compared to the conventional trench gate MOSFET. Furthermore, the graded strained accumulation region supports the confinement of carriers near the trench sidewalls improving the field distribution in the mesa structure useful for a better damage immunity during inductive switching.",1008.3019v1 2010-08-24,Dominant role of impurity scattering over crystalline anisotropy for magnetotransport properties in the quasi-1D Hollandite Ba1.2Rh8O16,"Angular magnetotransport measurements have been performed to tackle the origin of the magnetoresistance in the quasi-1D Hollandite Ba1.2Rh8O16. Three samples of different impurities amount were measured. We observe that the low temperature resistivity upturn is not due to a charge density wave transition, and a dominant role of impurities scattering for low temperature transport properties is instead demonstrated. The components of magnetoresistance were separated by using the Kohler plot and the angular dependency of the resistance under magnetic field. It shows the major contribution of an isotropic, likely spin driven, negative magnetoresistance. Galvanomagnetic characteristics are then consistent with a Kondo effect and appear to be essentially 3D at low temperature.",1008.4040v1 2010-09-27,Effect of vertex corrections on the longitudinal transport through multilayered nanostructures: Exact dynamical mean-field theory approach applied to the inhomogeneous Falicov-Kimball model,"Inhomogeneous dynamical mean-field theory is employed to calculate the vertex-corrected electronic charge transport for multilayered devices composed of semi-infinite metallic lead layers coupled through a strongly correlated material barrier region. The barrier region can be tuned from a metal to a Mott insulator through adjusting the interaction strength and the particle filling. We use the Falicov-Kimball model to describe the barrier region because an exact expression for the vertex corrections is known, allowing us to determine their effect on transport. The dc conductivity is calculated and we find the effects of the vertex corrections are relatively small, manifesting themselves in a small reduction in the resistance-area product. This reduction saturates in absolute magnitude as the barrier layer becomes thick, as expected due to the vanishing nature of the vertex corrections in bulk. The vertex corrections have a larger relative effect on the resistance-area product for more metallic and thinner devices.",1009.5299v1 2010-10-08,"A unified first-principles study of Gilbert damping, spin-flip diffusion and resistivity in transition metal alloys","Using a formulation of first-principles scattering theory that includes disorder and spin-orbit coupling on an equal footing, we calculate the resistivity $\rho$, spin flip diffusion length $l_{sf}$ and the Gilbert damping parameter $\alpha$ for Ni$_{1-x}$Fe$_x$ substitutional alloys as a function of $x$. For the technologically important Ni$_{80}$Fe$_{20}$ alloy, permalloy, we calculate values of $\rho = 3.5 \pm 0.15$ $\mu$Ohm-cm, $l_{sf}=5.5 \pm 0.3$ nm, and $\alpha= 0.0046 \pm 0.0001$ compared to experimental low-temperature values in the range $4.2-4.8$ $\mu$Ohm-cm for $\rho$, $5.0-6.0$ nm for $l_{sf}$, and $0.004-0.013$ for $\alpha$ indicating that the theoretical formalism captures the most important contributions to these parameters.",1010.1626v3 2010-10-23,Silicon Oxide is a Non-Innocent Surface for Molecular Electronics and Nanoelectronics Studies,"Silicon oxide (SiOx) has been widely used in many electronic systems as a supportive and insulating medium. Here we demonstrate various electrical phenomena such as negative differential resistance, resistive switching and current hysteresis intrinsic to a thin layer of SiOx. These behaviors can largely mimic numerous electrical phenomena observed in molecules and other nanomaterials, suggesting that substantial caution should be paid when studying conduction in electronic systems with SiOx as a component. The actual switching can be the result of SiOx and not the presumed molecular or nanomaterial component. These electrical properties and the underlying mechanisms are discussed in detail.",1010.4853v1 2010-11-17,Oxidation resistance of graphene-coated Cu and Cu/Ni alloy,"The ability to protect refined metals from reactive environments is vital to many industrial and academic applications. Current solutions, however, typically introduce several negative effects, including increased thickness and changes in the metal physical properties. In this paper, we demonstrate for the first time the ability of graphene films grown by chemical vapor deposition to protect the surface of the metallic growth substrates of Cu and Cu/Ni alloy from air oxidation. SEM, Raman spectroscopy, and XPS studies show that the metal surface is well protected from oxidation even after heating at 200 \degree C in air for up to 4 hours. Our work further shows that graphene provides effective resistance against hydrogen peroxide. This protection method offers significant advantages and can be used on any metal that catalyzes graphene growth.",1011.3875v1 2010-12-20,Conduction Electron Scattering and Spin-Flipping at Sputtered Co/Ni Interfaces,"Current-perpendicular-to-plane magnetoresistance (CPP-MR) measurements let us quantify conduction electron scattering and spin-flipping at a sputtered ferromagnetic/ferromagnetic (F1/F2 = Co/Ni) interface, with important consequences for CPP-MR and spin-torque experiments with perpendicular anisotropy. We use ferromagnetically coupled ([Ni/Co]xn)Ni multilayers, and Py-based, symmetric double exchange-biased spin-valves (DEBSVs) containing inserts of ferromagnetically coupled ([Co/Ni]xn)Co or ([Ni/Co]xn)Ni multilayers, to derive Co/Ni interface specific resistances AR(Co/Ni)(Up) = 0.03 (+0.02)(-0.03) f-ohm-m^2 and AR(Co/Ni)(down) = 1.00 +/- 0.07 f-ohm-m^2, and interface spin-flipping parameter delta(Co/Ni) = 0.35 +/- 0.05. The specific resistances are consistent with our no-free-parameter calculations for an interface thickness between 2 and 4 monolayers (ML) that is compatible with expectations.",1012.4388v1 2011-01-19,Negative differential resistance in scanning tunneling microscopy: simulations on C$_{60}$-based molecular overlayers,"We determine the conditions in which negative differential resistance (NDR) appears in the C$_{60}$-based molecular device of [Phys. Rev. Lett. {\bf 100}, 036807 (2008)] by means of ab-initio electron-transport simulations. Our calculations grant access to bias-dependent intrinsic properties of the molecular device, such as electronic levels and their partial widths. We show that these quantities depend on the molecule-molecule and molecule-electrode interactions of the device. Hence, NDR can be tuned by modifying the bias behavior of levels and widths using both types of interactions.",1101.3714v1 2011-01-26,Metal-insulator transition in ultrathin LaNiO3 films,"Transport in ultrathin films of LaNiO3 evolves from a metallic to a strongly localized character as the film's thickness is reduced and the sheet resistance reaches a value close to h/e2, the quantum of resistance in two dimensions. In the intermediate regime, quantum corrections to the Drude low- temperature conductivity are observed; they are accurately described by weak localization theory. Remarkably, the negative magnetoresistance in this regime is isotropic, which points to magnetic scattering associated with the proximity of the system to either a spin glass state or the charge ordered antiferromagnetic state observed in other rare earth nickelates.",1101.5111v2 2011-03-31,Aharonov-Casher effect in Bi$_{\rm 2}$Se$_{\rm 3}$ square-ring interferometers,"Electrical control of spin dynamics in Bi$_{\rm 2}$Se$_{\rm 3}$ was investigated in ring-type interferometers. Aharonov-Bohm and Altshuler-Aronov-Spivak resistance oscillations against magnetic field, and Aharorov-Casher resistance oscillations against gate voltage were observed in the presence of a Berry phase of $\pi$. A very large tunability of spin precession angle by gate voltage has been obtained, indicating that Bi$_{\rm 2}$Se$_{\rm 3}$-related materials with strong spin-orbit coupling are promising candidates for constructing novel spintronic devices.",1103.6115v1 2011-06-02,Evidence for semiconducting behavior with a narrow band gap of Bernal graphite,"We have studied the resistivity of a large number of highly oriented graphite samples with areas ranging from several mm$^2$ to a few $\mu$m$^2$ and thickness from $\sim 10 $nm to several tens of micrometers. The measured resistance can be explained by the parallel contribution of semiconducting graphene layers with low carrier density $< 10^9$ cm$^{-2}$ and the one from metallic-like internal interfaces. The results indicate that ideal graphite with Bernal stacking structure is a narrow-gap semiconductor with an energy gap $E_g \sim 40 $meV.",1106.0437v3 2011-07-25,Unveiling a nematic quantum critical point in multi-orbital systems,"Electronic nematicity, proposed to exist in a number of transition metal materials, can have different microscopic origins. In particular, the anisotropic resistivity and meta-magnetic jumps observed in Sr3Ru2O7 are consistent with an earlier proposal that the isotropic-nematic transition is generically first order and accompanied by meta-magnetism when tuned by a magnetic field. However, additional striking experimental features such as a non-Fermi liquid resistivity and critical thermodynamic behavior imply the presence of an unidentified quantum critical point (QCP). Here we show that orbital degrees of freedom play an essential role in revealing a nematic QCP, even though it is overshadowed by a nearby meta-nematic transition at low temperature. We further present a finite temperature phase diagram including the entropy landscape and discuss our findings in light of the phenomena observed in Sr3Ru2O7.",1107.5052v5 2011-08-25,Structural and Electrical Characterization of Bi2Se3 Nanostructures Grown by Metalorganic Chemical Vapor Deposition,"We characterize nanostructures of Bi2Se3 that are grown via metalorganic chemical vapor deposition using the precursors diethyl selenium and trimethyl bismuth. By adjusting growth parameters, we obtain either single-crystalline ribbons up to 10 microns long or thin micron-sized platelets. Four-terminal resistance measurements yield a sample resistivity of 4 mOhm-cm. We observe weak anti-localization and extract a phase coherence length l_phi = 178 nm and spin-orbit length l_so = 93 nm at T = 0.29 K. Our results are consistent with previous measurements on exfoliated samples and samples grown via physical vapor deposition.",1108.4978v2 2011-09-14,Growth of atomically smooth thin films of the electronically phase separated manganite (La$_{0.5}$Pr$_{0.5}$)$_{0.67}$Ca$_{0.33}$MnO$_{3}$,"Atomically flat, epitaxial, and stoichiometric thin films of the electronically phase separated compound (La$_{0.5}$Pr$_{0.5}$)$_{0.67}$Ca$_{0.33}$MnO$_{3}$ were grown on as-received and treated NdGaO$_{3}$ substrates by fine tuning of oxygen pressure during deposition. Optimal thin films with step flow growth mode show superior physical properties compared to thin films grown in off-optimal oxygen pressures, {\em viz.} the highest maximum temperature coefficient of resistance, the highest peak-resistivity temperature, and reduced coercive fields. Transport, magnetization, and x-ray diffraction measurements indicate that the oxygen pressure during growth plays a critical role in the formation of oxygen vacancies, cation vacancies, and grain boundaries.",1109.3225v1 2011-09-23,A single layer hydrogen silsesquioxane (HSQ) based lift-off process for germanium and platinum,"Primarily used as etch mask, single layer hydrogen silsesquioxane has never been investigated for lift-off technique. In this article, we propose a new technique where a single layer of hydrogen silsesquioxane, a negative tone electron beam resist, is used to make lift-off of germanium and platinum. Removal of exposed hydrogen silsesquioxane is tested for various concentrations of hydrofluoric acid. Ultrasonic agitation is also used to reduce the formation of flakes due to accumulation of matter (evaporated metal in our case) along the sidewalls of the lift-off narrow slots. Results demonstrate potential in applying the hydrogen silsesquioxane as a negative tone lift-off resist to pattern nanometer scale features into germanium and platinum layers.",1109.5187v1 2011-11-03,Estimation of the spin polarization for Heusler-compound thin films by means of nonlocal spin-valve measurements: Comparison of Co$_{2}$FeSi and Fe$_{3}$Si,"We study room-temperature generation and detection of pure spin currents using lateral spin-valve devices with Heusler-compound electrodes, Co$_{2}$FeSi (CFS) or Fe$_{3}$Si (FS). The magnitude of the nonlocal spin-valve (NLSV) signals is seriously affected by the dispersion of the resistivity peculiarly observed in the low-temperature grown Heusler compounds with ordered structures. From the analysis based on the one-dimensional spin diffusion model, we find that the spin polarization monotonically increases with decreasing the resistivity, which depends on the structural ordering, for both CFS and FS electrodes, and verify that CFS has relatively large spin polarization compared with FS.",1111.0742v2 2011-11-27,A first-order magnetic phase transition near 15 K with novel magnetic-field-induced effects in Er5Si3,"We present magnetic characterization of a binary rare-earth intermetallic compound Er5Si3, crystallizing in Mn5Si3-type hexagonal structure, through magnetization, heat-capacity, electrical resistivity, and magnetoresistance measurements. Our investigations confirm that the compound exhibits two magnetic transitions with decreasing temperature, first one at 35 K and the second one at 15 K. The present results reveal that the second magnetic transition is a disorder-broadened first-order transition, as shown by thermal hysteresis in the measured data. Another important finding is that, below 15 K, there is a magnetic-field-induced transition with a hysteretic effect with the electrical resistance getting unusually enhanced at this transition and the magnetorsistance (MR) is found to exhibit intriguing magnetic-field dependence indicating novel magnetic phase-co-existence phenomenon. It thus appears that this compound is characterized by interesting magnetic anomalies in the temperature-magnetic-field phase diagram.",1111.6240v1 2011-12-20,Approximate Theory of Temperature Coefficient of Resistivity of Amorphous Semiconductors,"In this paper, we develop an approximate theory of the temperature coefficient of resistivity (TCR) and conductivity based upon the recently proposed Microscopic Response Method. By introducing suitable approximations for the lattice dynamics, localized and extended electronic states, we produce new explicit forms for the conductivity and TCR, which depend on easily accessible material parameters. The theory is in reasonable agreement with experiments on a-Si:H and a-Ge:H. A long-standing puzzle, a \textquotedblleft kink\textquotedblright\ in the experimental $% \log_{10}\sigma $ vs. 1/T curve, is predicted by the theory and attributed to localized to extended transitions, which have not been properly handled in earlier theories.",1112.4723v2 2011-12-23,Microscopic Details of the Integer Quantum Hall Effect in an Anti-Hall Bar,"Due to the lack of simulation tools that take into account the actual geometry of complicated quantum Hall samples there are lots of experiments that are not yet fully understood. Already some years ago R. G. Mani recorded a shift of the Hall resistance transitions to lower magnetic fields in samples of a Hall bar with embedded anti-Hall bar by using partial gating. We use a Nonequilibrium Network Model (NNM) to simulate this geometry and find qualitative agreement. Fitting the simulated resistance curves to the experimental results we can not only determine the carrier concentration but also obtain an estimate of the screened gating potential and especially the amplitude and lengthscale of potential fluctuations from charge inhomogenities which are not easily accessible by experiment.",1112.5673v1 2012-02-27,Coaxial Nanowire Resonant Tunneling Diodes from non-polar AlN/GaN on Silicon,"Resonant tunneling diodes are formed using AlN/GaN core-shell nanowire heterostructures grown by plasma assisted molecular beam epitaxy on n-Si(111) substrates. By using a coaxial geometry these devices take advantage of non-polar (m-plane) nanowire sidewalls. Device modeling predicts non-polar orientation should enhance resonant tunneling compared to a polar structure and that AlN double barriers will lead to higher peak-to-valley current ratios compared to AlGaN barriers. Electrical measurements of ensembles of nanowires show negative differential resistance appearing only at cryogenic temperature. Individual nanowire measurements show negative differential resistance at room temperature with peak current density of 5*10^5 A/cm^2.",1202.6052v2 2012-04-09,Magnetic-field induced resistivity minimum with in-plane linear magnetoresistance of the Fermi liquid in SrTiO3-x single crystals,"We report novel magnetotransport properties of the low temperature Fermi liquid in SrTiO3-x single crystals. The classical limit dominates the magnetotransport properties for a magnetic field perpendicular to the sample surface and consequently a magnetic-field induced resistivity minimum emerges. While for the field applied in plane and normal to the current, the linear magnetoresistance (MR) starting from small fields (< 0.5 T) appears. The large anisotropy in the transverse MRs reveals the strong surface interlayer scattering due to the large gradient of oxygen vacancy concentration from the surface to the interior of SrTiO3-x single crystals. Moreover, the linear MR in our case was likely due to the inhomogeneity of oxygen vacancies and oxygen vacancy clusters, which could provide experimental evidences for the unusual quantum linear MR proposed by Abrikosov [A. A. Abrikosov, Phys. Rev. B 58, 2788 (1998)].",1204.1901v1 2012-04-20,Size-dependent electronic-transport mechanism and sign reversal of magnetoresistance in Nd0.5Sr0.5CoO3,"A detailed investigation of electronic-transport properties of Nd0.5Sr0.5CoO3 has been carried out as a function of grain size ranging from micrometer order down to an average size of 28 nm. Interestingly, we observe a size induced metal-insulator transition in the lowest grain size sample while the bulk-like sample is metallic in the whole measured temperature regime. An analysis of the temperature dependent resistivity in the metallic regime reveals that the electron-electron interaction is the dominating mechanism while other processes like electron-magnon and electron-phonon scatterings are also likely to be present. The fascinating observation of enhanced low temperature upturn and minimum in resistivity on reduction of grain size is found due to electron-electron interaction (quantum interference effect). This effect is attributed to enhanced disorder on reduction of grain size. Interestingly, we observed a cross over from positive to negative magnetoresistance in the low temperature regime as the grain size is reduced. This observed sign reversal is attributed to enhanced phase separation on decreasing the grain size of the cobaltite.",1204.4572v1 2012-04-22,Anomalous ferromagnetism and non-Fermi-liquid behavior in the Kondo lattice CeRuSi2,"The structural, electronic and magnetic properties of the Kondo-lattice system CeRuSi2 are experimentally investigated and analyzed in the series of other ternary cerium compounds. This system is shown to be an excellent model system demonstrating coexistence of the Kondo effect and anomalous ferromagnetism with a small magnetic moment which is confirmed by magnetic and \mu SR measurements. Data on specific heat, resistivity and Seebeck coefficient are presented. Being deduced from the resistivity and specific heat data, the non-Fermi-liquid behavior is observed at low temperatures, which is unusual for a ferromagnetic Kondo system. A comparison with other magnetic Kondo lattices is performed.",1204.4903v3 2012-07-02,Evolution of the magnetism of Tb(Co_{x}Ni_{1-x})_{2}B_{2}C,"The magnetic properties of polycrystalline Tb(Co_{x}Ni_{1-x})_{2}B_{2}C (x=0.2,0.4,0.6,0.8) samples were probed by magnetization, specific heat, ac susceptibility, and resistivity techniques. For x{\neq}0.4, the obtained curves are consistent with the features expected for the corresponding magnetic modes, namely k_{1}=(0.55,0,0) at x=0; k_{2}=([nicefrac]\nicefrac{1}{2},0,[nicefrac]\nicefrac{1}{2}) at x= 0.2; k_{3}=(0,0,[nicefrac]\nicefrac{1}{3}) at x= 0.6, and k_{4}=(0,0,0) at x= 0.8 and 1. For x=0.4, even though the neutron diffraction indicates a k_{2} mode, but with a reduced magnetic moment, the magnetization, the ac susceptibility, and resistivity indicate two magnetic events; furthermore, deviation from Curie-Weiss behavior is observed below 150 K for this sample. These features, together with the evolution of both magnetic moment and critical temperature, are attributed to an interplay between competing magnetic couplings; for the particular x=0.4 case, additional factors such as crystalline electric field effects may be in operation.",1207.0519v1 2012-07-19,Mobility enhancement and highly efficient gating of monolayer MoS2 transistors with Polymer Electrolyte,"We report electrical characterization of monolayer molybdenum disulfide (MoS2) devices using a thin layer of polymer electrolyte consisting of poly(ethylene oxide) (PEO) and lithium perchlorate (LiClO4) as both a contact-barrier reducer and channel mobility booster. We find that bare MoS2 devices (without polymer electrolyte) fabricated on Si/SiO2 have low channel mobility and large contact resistance, both of which severely limit the field-effect mobility of the devices. A thin layer of PEO/ LiClO4 deposited on top of the devices not only substantially reduces the contact resistance but also boost the channel mobility, leading up to three-orders-of-magnitude enhancement of the field-effect mobility of the device. When the polymer electrolyte is used as a gate medium, the MoS2 field-effect transistors exhibit excellent device characteristics such as a near ideal subthreshold swing and an on/off ratio of 106 as a result of the strong gate-channel coupling.",1207.4824v1 2012-07-20,"Magnetic, magnetocaloric and magnetotransport properties of RSn_{1+x}Ge_{1-x} compounds (R=Gd, Tb, Er; x=0.1)","We have studied the magnetic, magnetocaloric and magnetotransport properties of RSn1+xGe1-x(R=Gd, Tb, Er; x=0.1) series by means of magnetization, heat capacity and resistivity measurements. It has been found that all the compounds crystallize in the orthorhombic crystal structure described by the centrosymmetric space group Cmcm (No. 63). The magnetic susceptibility and heat capacity data suggest that all the compounds are antiferromagnetic. Large negative values of {\theta}p in case of GdSn1.1Ge0.9 and TbSn1.1Ge0.9 indicate that strong antiferromagnetic interactions are involved, which is also reflected in the magnetization isotherms. On the other hand ErSn1.1Ge0.9 shows weak antiferromagnetic interaction. The heat capacity data have been analyzed by fitting the temperature dependence and the values of {\theta}D and {\gamma} have been estimated. Among these three compounds, ErSn1.1Ge0.9 shows considerable magnetic entropy change of 9.5 J/kg K and an adiabatic temperature change of 3.2 K for a field of 50 kOe. The resistivity data in different temperature regimes have been analyzed and the dominant contributions have been identified. All the compounds show small but positive magnetoresistance.",1207.4971v1 2012-07-30,The Effect of Electrode Size on Memristor Properties: An Experimental and Theoretical Study,"The width of the electrodes is not included in the current phenomenological models of memristance, but is included in the memory-conservation (mem-con) theory of memristance. An experimental study of the effect of changing the top electrode width was performed on titanium dioxide sol-gel memristors. It was demonstrated that both the on resistance, Ron, and the off resistance, Roff, decreased with increasing electrode size. The memory function part of the mem-con model could fit the relationship between Ron and electrode size. Similarly, the conservation function fits the change in Roff. The experimentally measured hysteresis did not fit the phenomenological model's predictions. Instead the size of the hysteresis increased with increasing electrode size, and correlated well to decreasing Ron.",1207.6933v1 2012-08-06,A Variant of the Point Defect Model for Passivity of Metals,"A variant of the point defect model originally enunciated by Macdonald and co-workers is advanced and its theoretical implications for the steady state current density, barrier layer thickness and the concentration of metal vacancy at the metal/film interface are deduced. The differences between the original point defect model and the present variant are also highlighted. The empirical parameters alpha and beta in the original point defect model are replaced with two physical parameters Rcont and Rhof which represent respectively the electronic contact resistance at the metal/film interface and the electronic resistivity of the oxide film. The present variant correctly describes the annihilation of the metal vacancies at the metal/film interface and also enforces the conservation of particle and defect volumes during the solid-state reactions leading to the natural inclusion of the famous Pilling-Bedsworth ratio RPB into the model. Diagnostics which help to check the model predictions with experiments are given. Use of this variant to describe stress-induced failure of the barrier oxide leading to pitting is also discussed.",1208.1096v1 2012-08-27,Suppression of superconductivity in layered Bi4O4S3 by Ag doping,"We report X-ray diffraction, magnetization and transport measurements for polycrystalline samples of the new layered superconductor Bi4-xAgxO4S3 (00.10. Accordingly, the resistivity changes from a metallic behavior for x<0.1 to a semiconductor-like behavior for x>0.1. The analysis of Seebeck coefficient shows there are two types of electron-like carriers dominate at different temperature regions, indicative of a multiband effect responsible for the transport properties. The suppression of superconductivity and the increased resistivity can be attributed to a shift of the Fermi level to the lower-energy side upon doping, which reduces the density of states at EF. Further, our result indicates the superconductivity in the parent Bi4O4S3 is intrinsic and the dopant Ag prefers to enter the BiS2 layers, which may essentially modify the electronic structure.",1208.5307v1 2012-09-27,Theoretical investigation of direct and phonon-assisted tunneling currents in InAlGaAs-InGaAs bulk and quantum well interband tunnel junctions for multi-junction solar cells,"Direct and phonon-assisted tunneling currents in InAlGaAs-InGaAs bulk and double quantum well interband tunnel heterojunctions are simulated rigorously using the non-equilibrium Green's function formalism for coherent and dissipative quantum transport in combination with a simple two-band tight-binding model for the electronic structure. A realistic band profile and associated built-in electrostatic field is obtained via self-consistent coupling of the transport formalism to Poisson's equation. The model reproduces experimentally observed features in the current-voltage characteristics of the device, such as the structure appearing in the negative differential resistance regime due to quantization of emitter states. Local maps of density of states and current spectrum reveal the impact of quasi-bound states, electric fields and electron-phonon scattering on the interband tunneling current. In this way, resonances appearing in the current through the double quantum well structure in the negative differential resistance regime can be related to the alignment of subbands in the coupled quantum wells.",1209.6314v1 2012-10-11,Prediction of semi-metallic tetragonal Hf2O3 and Zr2O3 from first-principles,"A tetragonal phase is predicted for Hf2O3 and Zr2O3 using density functional theory. Starting from atomic and unit cell relaxations of substoichiometric monoclinic HfO2 and ZrO2, such tetragonal structures are only reached at zero temperature by introducing the oxygen vacancy pair with the lowest formation energy. The tetragonal Hf2O3 and Zr2O3 structures belong to space group P-4m2 and are more stable than their corundum structure counterparts. These phases are semi-metallic, as confirmed through further G0W0 calculations. The carrier concentrations are estimated to be 1.77E21 cm^{-3} for both electrons and holes in tetragonal Hf2O3, and 1.75E21 cm^{-3} for both electrons and holes in tetragonal Zr2O3. The tetragonal Hf2O3 phase is probably related to the low resistivity state of hafnia-based resistive random access memory (RRAM).",1210.3348v1 2012-10-12,Superconducting LaAlO3/SrTiO3 Nanowires,"We report superconductivity in quasi-1D nanostructures created at the LaAlO3/SrTiO3 interface. Nanostructures having line widths w~10 nm are formed from the parent two-dimensional electron liquid using conductive atomic force microscope lithography. Nanowire cross-sections are small compared to the superconducting coherence length in LaAlO3/SrTiO3 (w<