TiO2 nanostructures were prepared by hydrothermal corrosion of Ti sheets for various heating temperatures and times. Their change from thick and short nanorods to thin and long nanowires by increasing these processing parameters led to improved photocatalytic properties.
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"title+abstract_embedding_113": -0.035944477, "title+abstract_embedding_114": -0.19529858, "title+abstract_embedding_115": -0.16970041, "title+abstract_embedding_116": -0.05580896, "title+abstract_embedding_117": 0.043210074, "title+abstract_embedding_118": -0.050970413, "title+abstract_embedding_119": -0.1936237, "title+abstract_embedding_120": -0.0270408, "title+abstract_embedding_121": -0.035268374, "title+abstract_embedding_122": 0.23308918, "title+abstract_embedding_123": -0.03532388, "title+abstract_embedding_124": 0.028647415, "title+abstract_embedding_125": -0.020486996, "title+abstract_embedding_126": -0.02581511, "title+abstract_embedding_127": -0.046405107, "label": 3, "label-multi": "3" }, { "paper_new_id": 5, "id": "j_0800179a645ade38c794bcfb5d7ec99c", "title+abstract": "Ina??Situ Activated NiFePBAa??FeOOH Electrocatalyst for Oxygen Evolution Reaction and Zinca??Air Battery;A cost-effective OER catalyst composing of nickel-iron Prussian blue analogues and iron oxyhydroxide (NiFePBA-FeOOH) prepared by facile hydrothermal method exhibits superior OER performance with low overpotential, small Tafel slope and steady durability, which is benefitting by the increasing specific surface area and accelerated charge transfer and the synergistic effect between in-situ activated nickel and ion oxyhydroxides.", "title+abstract_embedding_0": -1.4927027, "title+abstract_embedding_1": -0.5843403, "title+abstract_embedding_2": -0.28778544, "title+abstract_embedding_3": -0.2161324, "title+abstract_embedding_4": 0.6409518, "title+abstract_embedding_5": -0.9115075, "title+abstract_embedding_6": 0.22347955, "title+abstract_embedding_7": -0.025555402, "title+abstract_embedding_8": 0.07472837, "title+abstract_embedding_9": 0.49747184, "title+abstract_embedding_10": 0.18266967, "title+abstract_embedding_11": 0.4189881, "title+abstract_embedding_12": 0.11334416, "title+abstract_embedding_13": 0.43783852, "title+abstract_embedding_14": 0.045347035, "title+abstract_embedding_15": 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-0.048288018, "label": 3, "label-multi": "3" }, { "paper_new_id": 6, "id": "j_08b8582c9fc537a4d03145598faab96f", "title+abstract": "Poly(aniline-co-o-aminophenol) nanostructured network: Electrochemical controllable synthesis and electrocatalysis;Abstract Poly(aniline-co- o -aminophenol) (copolymer) with nanostructured network has been synthesized in the presence of ferrocenesulfonic acid, using repeated potential cycling between ?0.10 and 0.86?V (versus SCE). The sizes of the fibers in the nanostructures can be controlled by the number of the cycles during copolymerization. The presence of ferrocenesulfonic acid possessing a larger molecular size with positive charges is favorable for the formation of nanostructures. The SEM images reveal a fact that the copolymer films synthesized under different cycles are constructed of interwoven fibers with average diameters in a range of 70¡§C107?nm. The copolymer with the nanostructured network deposited on a platinum foil offers a convenient way to study directly the electrochemical property of nanostructures and can effectively catalyze the electrochemical oxidation of catechol in the Na 2 SO 4 solution with pH 5.0. It was found that the electrochemical oxidation of catechol was affected by the sizes of the copolymer fibers. Evidence is that its anodic peak potential increases with increasing the diameter of the fibers in the nanostructures. The copolymer synthesized in the presence of ferrocenesulfonic acid has a good electrochemical activity at pH??¨¹?9.0, a larger usable potential window and faster electron transfer ability compared with the copolymer synthesized in the absence of ferrocenesulfonic acid.", "title+abstract_embedding_0": 0.58014023, "title+abstract_embedding_1": -1.0278254, "title+abstract_embedding_2": -0.07672945, "title+abstract_embedding_3": 0.051334858, "title+abstract_embedding_4": -0.63344705, "title+abstract_embedding_5": 0.4277193, "title+abstract_embedding_6": -0.3812975, "title+abstract_embedding_7": 0.063304044, "title+abstract_embedding_8": -0.122573845, "title+abstract_embedding_9": -0.23958641, "title+abstract_embedding_10": 0.22948337, "title+abstract_embedding_11": -0.33086765, "title+abstract_embedding_12": -0.1343329, "title+abstract_embedding_13": -0.108017914, "title+abstract_embedding_14": 0.30233207, "title+abstract_embedding_15": 0.12958343, "title+abstract_embedding_16": 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"paper_new_id": 7, "id": "j_094fa294e21f65c8dcfc76a451d08a77", "title+abstract": "(I2)n Encapsulation inside TiO2:a?? A Way To Tune Photoactivity in the Visible Region;We report on the synthesis of nanovoid-structured TiO(2) material via a sol-gel route using titanium isopropoxide as precursor. The nanovoids are formed during the thermal treatment in air at 773 K. The surfaces of internal cavities are populated by the partial oxidation products of the organic part of the Ti precursor (CO(2), hydrogen carbonates, and residual isopropoxide groups). The thermal treatment in air at 773 K allows the maintainence, in the internal voids, of the encapsulated species. Addition of iodine in the synthesis procedure results in a new nanovoid-structured titanium oxide able to absorb light in the whole visible part of the electromagnetic spectrum. The origin of this absorption is attributed to the presence of (I(2))(n) adducts encapsulated in the nanocavities. These species coexist with partial combustion products of isopropoxide groups. Due to the protection of the TiO(2) walls, the (I(2))(n) adducts are not destroyed by thermal treatments in air. We have investigated whether the electron promoted in the excited state of the dye molecule (upon absorption of visible light from the (I(2))(n) adducts) can be injected into either the TiO(2) conduction band or some titanium-localized acceptor, followed by migration of the injected electron to the surface where it reduces adsorbed organic molecules. Preliminarily experiments conducted with sunlight show that the surface-specific efficiency of this process, tested by following the degradation of methylene blue, is about 10 times higher than that of the P25 commercial TiO(2) photocatalyst.", "title+abstract_embedding_0": 0.75855744, "title+abstract_embedding_1": -0.22375074, "title+abstract_embedding_2": 0.055072993, "title+abstract_embedding_3": 0.5716962, "title+abstract_embedding_4": 0.3100142, "title+abstract_embedding_5": 0.5131015, "title+abstract_embedding_6": 0.024819195, "title+abstract_embedding_7": 0.014340535, "title+abstract_embedding_8": -0.20840262, "title+abstract_embedding_9": -0.23978478, "title+abstract_embedding_10": -0.18189158, "title+abstract_embedding_11": -0.33047423, "title+abstract_embedding_12": 0.15897799, "title+abstract_embedding_13": 0.22217336, "title+abstract_embedding_14": 0.18535104, "title+abstract_embedding_15": 0.24616288, "title+abstract_embedding_16": -0.38276473, 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"id": "j_0a40fd9b0a305baea7fb88857a72862b", "title+abstract": "Investigation of the Role of Ionic Liquids in Imparting Electrocatalytic Behavior to Carbon Paste Electrode;In this paper, a survey has been undertaken to clarify the possible reasons for the electrocatalytic activity obtained by the presence of ionic liquid in carbon paste electrode (CPE). For this purpose, the effect of the addition of traces of ionic liquid to conventional CPE was investigated. Fe(CN)63?/4? was used as a probe and two ionic liquids, namely n-octylpyridinum hexafluorophosphate and 1-octyl-3-methylimidazolium hexaflourophosphate were tested for their electrocatalytic activity. The reasons for this electrocatalytic behavior were evaluated and it was found that different factors such as increase in the ionic conduction of the binder, decrease in the resistance of the modified electrode, increase in ion exchange properties of the electrode and the inherent catalytic activity of ionic liquids are responsible for the considerable improved electrochemical response obtained in the presence of traces of ionic liquid.", "title+abstract_embedding_0": -0.84794235, "title+abstract_embedding_1": -0.97965944, "title+abstract_embedding_2": 0.5633194, "title+abstract_embedding_3": 1.1192814, "title+abstract_embedding_4": 0.11135334, "title+abstract_embedding_5": -0.24938184, "title+abstract_embedding_6": 0.30628717, "title+abstract_embedding_7": -0.004234336, "title+abstract_embedding_8": -0.5367482, "title+abstract_embedding_9": -0.15227985, "title+abstract_embedding_10": 0.7766871, "title+abstract_embedding_11": 0.15978473, "title+abstract_embedding_12": -0.016198963, 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"title+abstract_embedding_126": 0.16116099, "title+abstract_embedding_127": 0.07885806, "label": 3, "label-multi": "14;3" }, { "paper_new_id": 9, "id": "j_0b4b7b3ea05e8ea2344fead3b5e5de50", "title+abstract": "Polymeric hybrid films with photocatalytic activity under visible light;nan", "title+abstract_embedding_0": -1.6061509, "title+abstract_embedding_1": 2.286634, "title+abstract_embedding_2": -1.2096024, "title+abstract_embedding_3": -0.6532302, "title+abstract_embedding_4": -0.81373954, "title+abstract_embedding_5": -0.2866451, "title+abstract_embedding_6": -0.075286865, "title+abstract_embedding_7": 0.37215355, "title+abstract_embedding_8": -0.544298, "title+abstract_embedding_9": -1.0024692, "title+abstract_embedding_10": 0.17877758, "title+abstract_embedding_11": 0.05694887, "title+abstract_embedding_12": -0.45325086, "title+abstract_embedding_13": -0.41688594, "title+abstract_embedding_14": 0.4412445, "title+abstract_embedding_15": 1.5647494, "title+abstract_embedding_16": 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"title+abstract_embedding_108": -0.059822414, "title+abstract_embedding_109": -0.040864393, "title+abstract_embedding_110": -0.20502786, "title+abstract_embedding_111": -0.2196897, "title+abstract_embedding_112": 0.17403859, "title+abstract_embedding_113": 0.22400594, "title+abstract_embedding_114": 0.14354613, "title+abstract_embedding_115": 0.039212972, "title+abstract_embedding_116": -0.007892497, "title+abstract_embedding_117": 0.08158359, "title+abstract_embedding_118": 0.06971809, "title+abstract_embedding_119": -0.31965333, "title+abstract_embedding_120": 0.16591707, "title+abstract_embedding_121": 0.021013623, "title+abstract_embedding_122": 0.025717184, "title+abstract_embedding_123": -0.16554466, "title+abstract_embedding_124": 0.001495935, "title+abstract_embedding_125": 0.1660851, "title+abstract_embedding_126": -0.059249826, "title+abstract_embedding_127": 0.14614251, "label": 21, "label-multi": "21" }, { "paper_new_id": 10, "id": "j_0b9596793e2594b2be33d7dcb65197c5", "title+abstract": "Facile Synthesis of Graphene Aerogel Supported Nickel/Nickel Oxide Corea??Shell Nanoparticles: Efficient Electrocatalysts for Oxygen Evolution Reactions;Graphene aerogels decorated with nickel/nickel oxide core¡§Cshell nanoparticles are synthesized via a one-pot hydrothermal reaction followed by thermal reduction. Nickel loading is varied from 1.5 to 40 wt % in a highly controlled fashion by simply tuning Ni2+ to graphene oxide ratio in the hydrothermal reaction mixture. In fact, graphene aerogel loaded with 40 wt % Ni has a BET surface area of 560 m2 g¡§C1 due to the preservation of the porous structure with the aid of supercritical CO2 drying. The thermal reduction applied for the growth of nanoparticles induces deoxygenation of graphene aerogel structure simultaneously. Valence band spectroscopy results reveal an increase in metallicity with a gradual increase in the nickel loading, which has a direct impact on the final electrocatalytic performance. For the evaluation of the electrocatalytic activity of Ni/NiO loaded aerogels toward oxygen evolution reaction, cyclic voltammetry (coupled with a rotating disk electrode) is utilized. In fact, 40 wt % Ni load...", "title+abstract_embedding_0": -0.08896315, "title+abstract_embedding_1": -0.8627046, "title+abstract_embedding_2": -0.7974287, "title+abstract_embedding_3": 0.16469818, "title+abstract_embedding_4": 0.16749781, "title+abstract_embedding_5": -0.24890679, "title+abstract_embedding_6": -0.29956302, "title+abstract_embedding_7": -0.55877376, "title+abstract_embedding_8": 0.14596206, "title+abstract_embedding_9": 0.03174588, "title+abstract_embedding_10": -0.16670993, "title+abstract_embedding_11": -0.22740398, "title+abstract_embedding_12": -0.335691, "title+abstract_embedding_13": -0.46138075, "title+abstract_embedding_14": 0.30198696, "title+abstract_embedding_15": 0.11718, "title+abstract_embedding_16": 0.21138892, "title+abstract_embedding_17": 0.18549219, "title+abstract_embedding_18": -0.06658177, "title+abstract_embedding_19": 0.68639266, "title+abstract_embedding_20": 0.5934296, "title+abstract_embedding_21": -0.23681626, "title+abstract_embedding_22": 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"title+abstract_embedding_113": -0.090197, "title+abstract_embedding_114": -0.10740675, "title+abstract_embedding_115": -0.03631822, "title+abstract_embedding_116": 0.09841007, "title+abstract_embedding_117": -0.015723586, "title+abstract_embedding_118": 0.15947026, "title+abstract_embedding_119": -0.11809322, "title+abstract_embedding_120": 0.004219294, "title+abstract_embedding_121": 0.24723788, "title+abstract_embedding_122": -0.16827741, "title+abstract_embedding_123": 0.036601454, "title+abstract_embedding_124": -0.11155743, "title+abstract_embedding_125": 0.078206666, "title+abstract_embedding_126": 0.018101383, "title+abstract_embedding_127": -0.06110449, "label": 3, "label-multi": "1;15;3" }, { "paper_new_id": 11, "id": "j_0cebfc8ac5c28d0dd844d409c77795ac", "title+abstract": "Low-temperature ozone treatment for carbon nanotube template removal: improving the template-based ALD method;This work addresses the production of stand-alone ceramic nanotubes by the template-based ALD method at low temperature. Nitrogen-doped multiwalled carbon nanotubes (CNTs) were coated with ZnO. Afterward, the template removal was evaluated by two different approaches: using oxidation in dry air or in an ozone-rich atmosphere. The samples treated by the two different methods were analyzed by XRD, TEM, SAED, and Raman spectroscopy. The dry air atmosphere requires high temperatures (~?700???C) for a complete CNT removal; at that temperature, the ZnO tubular shape is completely collapsed due to recrystallization. Under ozone atmosphere, the template can be removed at temperatures as low as 85???C; this temperature is lower than the ALD preparation temperature (120???C). The ozone treatment maintains the tubular shape of the ZnO nanostructures. Photocatalytic activity of the ZnO samples was evaluated using the photo-oxidation of Amaranth as probe reaction, showing a higher activity the ZnO nanotubes obtained from the low-temperature ozone treatment than the high-temperature processed materials. The use of ozone for the template removal reinforces the template-based ALD method to produce inorganic nanotubes.", "title+abstract_embedding_0": 0.26844203, "title+abstract_embedding_1": -0.19529632, "title+abstract_embedding_2": -0.1180968, "title+abstract_embedding_3": 0.46644652, "title+abstract_embedding_4": 0.017201543, "title+abstract_embedding_5": -0.7276875, "title+abstract_embedding_6": -0.34841993, "title+abstract_embedding_7": -0.12057762, "title+abstract_embedding_8": 0.9638161, "title+abstract_embedding_9": 0.42358252, "title+abstract_embedding_10": -0.66693306, "title+abstract_embedding_11": -0.61366355, "title+abstract_embedding_12": -0.23897746, "title+abstract_embedding_13": 0.5200576, "title+abstract_embedding_14": -0.058899894, "title+abstract_embedding_15": -0.000736566, "title+abstract_embedding_16": -0.26111588, "title+abstract_embedding_17": 0.38998362, "title+abstract_embedding_18": 0.33990008, "title+abstract_embedding_19": 0.1916495, 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"title+abstract_embedding_65": 0.06954105, "title+abstract_embedding_66": -0.08095137, "title+abstract_embedding_67": -0.3220556, "title+abstract_embedding_68": 0.004275128, "title+abstract_embedding_69": 0.023768786, "title+abstract_embedding_70": 0.21062878, "title+abstract_embedding_71": 0.040131107, "title+abstract_embedding_72": 0.13596877, "title+abstract_embedding_73": -0.035253696, "title+abstract_embedding_74": 0.1494029, "title+abstract_embedding_75": 0.17963928, "title+abstract_embedding_76": 0.06605378, "title+abstract_embedding_77": -0.050539568, "title+abstract_embedding_78": -0.08428231, "title+abstract_embedding_79": -0.20996076, "title+abstract_embedding_80": -0.30097955, "title+abstract_embedding_81": -0.15464959, "title+abstract_embedding_82": -0.104243904, "title+abstract_embedding_83": -0.057929598, "title+abstract_embedding_84": 0.058605775, "title+abstract_embedding_85": -0.15538132, "title+abstract_embedding_86": -0.21582502, "title+abstract_embedding_87": 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"title+abstract_embedding_110": 0.09214115, "title+abstract_embedding_111": 0.10016001, "title+abstract_embedding_112": 0.2016516, "title+abstract_embedding_113": 0.15792762, "title+abstract_embedding_114": 0.14365363, "title+abstract_embedding_115": -0.07180228, "title+abstract_embedding_116": 0.08269147, "title+abstract_embedding_117": -0.33703792, "title+abstract_embedding_118": -0.002525808, "title+abstract_embedding_119": 0.03934302, "title+abstract_embedding_120": -0.10244651, "title+abstract_embedding_121": -0.023168212, "title+abstract_embedding_122": 0.115774214, "title+abstract_embedding_123": 0.34096026, "title+abstract_embedding_124": -0.07932647, "title+abstract_embedding_125": 0.22118965, "title+abstract_embedding_126": -0.05723533, "title+abstract_embedding_127": -0.06357576, "label": 3, "label-multi": "1;15;3" }, { "paper_new_id": 12, "id": "j_0ea65abbbc1f77dc16f3e85fe7805793", "title+abstract": "Photocatalytic water splitting over Pt-loaded TiO2 (Pt/TiO2) catalysts prepared by the polygonal barrel-sputtering method;Abstract Pt-loaded TiO2 (Pt/TiO2) catalysts for photocatalytic water splitting were prepared by the polygonal barrel-sputtering method. The results showed that the evolution rates of H2 and O2 gases for our Pt/TiO2 catalysts were ca. 5¡§C10 times of those prepared by a conventional photodeposition method. The molar ratios of H2 versus O2 were close to be 2, revealing that the stoichiometric water decomposition occurred. The characterizations of the prepared samples implied that the smaller Pt nanoparticles were highly dispersed on the TiO2 particles by the polygonal barrel-sputtering method. The deposition of the smaller Pt particles increased the Pt surface areas, which can improve the water splitting activities. In addition, the particles deposited by the sputtering method were electron-de?cient Pt metals that can enhance the water splitting reaction, whereas those by the photodeposition method were electron-rich Pt metals that reduce the effectiveness of the photocatalytic reaction. These different electron states would play an important role in the remarkable differences in the water splitting activities between the Pt/TiO2 catalysts. Consequently, the polygonal barrel-sputtering method is useful for preparing photocatalysts with the high water splitting activities.", "title+abstract_embedding_0": 0.37833095, "title+abstract_embedding_1": 0.55845594, "title+abstract_embedding_2": 0.13572842, "title+abstract_embedding_3": -0.008011341, "title+abstract_embedding_4": 0.605861, "title+abstract_embedding_5": 0.53630495, "title+abstract_embedding_6": 0.011541158, "title+abstract_embedding_7": -0.45090118, "title+abstract_embedding_8": 0.11336542, "title+abstract_embedding_9": 0.020769596, "title+abstract_embedding_10": -0.8025812, "title+abstract_embedding_11": -0.112581424, "title+abstract_embedding_12": 0.17435935, "title+abstract_embedding_13": -0.20365489, "title+abstract_embedding_14": 0.3282731, "title+abstract_embedding_15": -0.24771857, "title+abstract_embedding_16": 0.42203587, "title+abstract_embedding_17": -0.022078395, "title+abstract_embedding_18": 0.3844117, "title+abstract_embedding_19": -0.26912805, 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"title+abstract_embedding_111": 0.035305828, "title+abstract_embedding_112": -0.09785338, "title+abstract_embedding_113": 5.6117773e-05, "title+abstract_embedding_114": 0.03213699, "title+abstract_embedding_115": -0.05762703, "title+abstract_embedding_116": 0.045671497, "title+abstract_embedding_117": 0.07936958, "title+abstract_embedding_118": 0.033109054, "title+abstract_embedding_119": 0.010836367, "title+abstract_embedding_120": 0.10012461, "title+abstract_embedding_121": -0.019219985, "title+abstract_embedding_122": -0.038806945, "title+abstract_embedding_123": -0.03846457, "title+abstract_embedding_124": 0.065648556, "title+abstract_embedding_125": -0.09275513, "title+abstract_embedding_126": 0.009651184, "title+abstract_embedding_127": -0.10874595, "label": 3, "label-multi": "0;3" }, { "paper_new_id": 13, "id": "j_100f0d8ed2f26f7f5525b85f1f6a5ed6", "title+abstract": "Effect of dissolved silica on photocatalytic water purification with a TiO2 ceramic catalyst;If photocatalytic water purification technologies will find practical applications, the impact of total dissolved solids in the source water on the activity of the photocatalyst must be evaluated. In this study, we evaluated the effects of SiO32- in water on a TiO2 ceramic photocatalyst; specifically, we determined the effects of SiO32- on the rate of photocatalytic degradation of formic acid (as a model contaminant) and on the rate of photocatalytic inactivation of Escherichia coli in an aqueous solution. Both the rate of formic acid degradation and the sterilization rate decreased with increasing SiO32- concentration. On the other hand, at a given SiO32- concentration, the activity of the photocatalyst did not decrease over the course of 120?h, and the surface structure of the photocatalyst did not change (i.e., no precipitate formed on the surface). The decreases in photocatalytic activity due to the presence of SiO32- could be recovered by flushing the experimental apparatus with distilled water. These results show that the reason for the lower photocatalytic activity in the presence of SiO32- than in its absence was due to adsorption of SiO32- onto the surface of the TiO2 photocatalyst and that SiO32- adsorption was an equilibrium process in water.", "title+abstract_embedding_0": 0.53330874, "title+abstract_embedding_1": 1.2066374, "title+abstract_embedding_2": 0.6699302, "title+abstract_embedding_3": 0.15325063, "title+abstract_embedding_4": 0.41706735, "title+abstract_embedding_5": 0.034308076, "title+abstract_embedding_6": -0.24752101, "title+abstract_embedding_7": -0.37764266, "title+abstract_embedding_8": -0.51916915, "title+abstract_embedding_9": 0.15202332, "title+abstract_embedding_10": -0.11595029, "title+abstract_embedding_11": 0.06915416, "title+abstract_embedding_12": 0.20879778, "title+abstract_embedding_13": 0.20894271, "title+abstract_embedding_14": 0.15205544, "title+abstract_embedding_15": -0.054482758, "title+abstract_embedding_16": 0.53379226, 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"id": "j_10744c3d5b71ef3949c7036ed05d7ec9", "title+abstract": "A bifunctional and stable Nia??Coa??S/Nia??Coa??P bistratal electrocatalyst for 10.8%-efficient overall solar water splitting;A bifunctional NiCoS/NiCoP catalyst with bistratal structure for 10.8%-efficient and stable overall solar water splitting.
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"title+abstract_embedding_113": 0.0483364, "title+abstract_embedding_114": -0.08298799, "title+abstract_embedding_115": 0.015604578, "title+abstract_embedding_116": -0.28091127, "title+abstract_embedding_117": -0.021673717, "title+abstract_embedding_118": 0.016445603, "title+abstract_embedding_119": 0.10267593, "title+abstract_embedding_120": 0.111083776, "title+abstract_embedding_121": -0.16132656, "title+abstract_embedding_122": 0.028917134, "title+abstract_embedding_123": 0.069944434, "title+abstract_embedding_124": -0.049220614, "title+abstract_embedding_125": -0.17771861, "title+abstract_embedding_126": 0.02068099, "title+abstract_embedding_127": 0.060805075, "label": 3, "label-multi": "1;17;3" }, { "paper_new_id": 15, "id": "j_12c982c046cbe395239b57741aaa26f4", "title+abstract": "Nanospherical Carbon Nitride Frameworks with Sharp Edges Accelerating Charge Collection and Separation at a Soft Photocatalytic Interface;Shape engineering of a g-C3 N4 framework, with interconnecting nanosheets and highly open-up spherical surfaces with sharp edges, can easily accelerate charge separation and promote mass transfer for photoredox catalysis, achieving an apparent quantum yield of 9.6% at 420 nm in an assay of the photocatalytic hydrogen evolution reaction.", "title+abstract_embedding_0": -1.800009, "title+abstract_embedding_1": 0.70342994, "title+abstract_embedding_2": -0.7534517, "title+abstract_embedding_3": -0.74033284, "title+abstract_embedding_4": -0.8072515, "title+abstract_embedding_5": 0.16641912, "title+abstract_embedding_6": 0.3201483, "title+abstract_embedding_7": -0.8231875, "title+abstract_embedding_8": -0.014502673, "title+abstract_embedding_9": -0.025192678, "title+abstract_embedding_10": 0.1358298, "title+abstract_embedding_11": -0.22767843, "title+abstract_embedding_12": -0.30935505, "title+abstract_embedding_13": 0.3371169, "title+abstract_embedding_14": 0.41776308, "title+abstract_embedding_15": -0.028574448, "title+abstract_embedding_16": 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"j_12e6355f0ce2db067740a9ea2c6609c7", "title+abstract": "TiO2 Nanotubes for Solar Water Splitting: Vacuum Annealing and Zr Doping Enhance Water Oxidation Kinetics;Herein, we report the cooperative effect of Zr doping and vacuum annealing on the carrier dynamics and interfacial kinetics of anodized TiO2 nanotubes for light-driven water oxidation. After evaluation of different Zr loads and different annealing conditions, it was found that both Zr doping and vacuum annealing lead to a significantly enhanced light harvesting efficiency and photoelectrochemical performance. The substitution of Zr4+ by Ti4+ species leads to a higher density of surface defects such as oxygen vacancies, facilitating electron trapping on Zr4+, which reduced the charge recombination and hence boosted the charge transfer kinetics. More importantly, vacuum annealing promoted the presence of surface defects. Furthermore, the mechanistic study through impedance spectroscopy revealed that both charge transfer and surface conductivity are significantly enhanced due the presence of an oxygen-deficient TiO2 surface. These results represent an important step forward in the optimization of nanostructured TiO2-based photoelectrodes, with high potential in photocatalytic applications, including solar fuel production.", "title+abstract_embedding_0": 0.005573034, "title+abstract_embedding_1": 0.41934824, "title+abstract_embedding_2": -0.6581937, "title+abstract_embedding_3": 0.2562095, "title+abstract_embedding_4": 0.09312165, "title+abstract_embedding_5": -0.5034183, "title+abstract_embedding_6": 0.30124104, "title+abstract_embedding_7": -0.82837224, "title+abstract_embedding_8": -0.19045357, "title+abstract_embedding_9": 0.14901724, "title+abstract_embedding_10": -0.54305995, "title+abstract_embedding_11": -0.277503, "title+abstract_embedding_12": 0.2373428, "title+abstract_embedding_13": 0.020426381, "title+abstract_embedding_14": -0.14785996, "title+abstract_embedding_15": -0.51224506, "title+abstract_embedding_16": -0.5166049, "title+abstract_embedding_17": -0.2176785, 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"title+abstract_embedding_108": -0.14136845, "title+abstract_embedding_109": -0.02267465, "title+abstract_embedding_110": -0.05738741, "title+abstract_embedding_111": 0.21380499, "title+abstract_embedding_112": -0.037658766, "title+abstract_embedding_113": 0.14759482, "title+abstract_embedding_114": 0.029090002, "title+abstract_embedding_115": 0.16198705, "title+abstract_embedding_116": 0.059989393, "title+abstract_embedding_117": 0.090021044, "title+abstract_embedding_118": 0.08289409, "title+abstract_embedding_119": -0.09712143, "title+abstract_embedding_120": -0.043080855, "title+abstract_embedding_121": 0.053612337, "title+abstract_embedding_122": 0.20353264, "title+abstract_embedding_123": -0.009921022, "title+abstract_embedding_124": 0.18112932, "title+abstract_embedding_125": -0.02132821, "title+abstract_embedding_126": 0.063799694, "title+abstract_embedding_127": -0.043022707, "label": 3, "label-multi": "3" }, { "paper_new_id": 17, "id": "j_137103c41335d9a9cd88d22aa41491b5", "title+abstract": "Morphogenesis of Highly Ordered Mixed-Valent Mesoporous Molybdenum Oxides;Control of the size, shape, and structure of mesoporous transition metal oxide materials is important in their correlations with corresponding optoelectronic and photocatalytic properties. Highly ordered cubic phases of mixed-valent mesoporous molybdenum oxides have been prepared by the reduction and decomposition of aqueous molybdenum precursor solution in the presence of poly(ethylene oxide) under ultrasonic irradiation. Large-scale uniform molybdenum oxide particles with well-defined crystal-like morphologies (ball-like, rhombic dodecahedral, and cubic shapes) were synthesized and found to be controllable by modifying the molecular chain length of the polymeric additive. Molybdenum oxides with an average oxidation state of 4.8 form a cubic lattice of open mesoporous structures.", "title+abstract_embedding_0": 0.097905874, "title+abstract_embedding_1": -0.45581096, "title+abstract_embedding_2": 0.106372416, "title+abstract_embedding_3": -0.014278054, "title+abstract_embedding_4": -0.4708446, "title+abstract_embedding_5": 0.5486617, "title+abstract_embedding_6": 0.25572354, "title+abstract_embedding_7": 0.71911025, "title+abstract_embedding_8": 0.076611996, "title+abstract_embedding_9": 0.57455397, "title+abstract_embedding_10": 0.20677891, "title+abstract_embedding_11": -0.22015838, "title+abstract_embedding_12": -0.4290698, "title+abstract_embedding_13": 0.007888168, "title+abstract_embedding_14": 0.31578258, "title+abstract_embedding_15": -0.43290222, "title+abstract_embedding_16": 0.03160122, "title+abstract_embedding_17": -0.22679502, "title+abstract_embedding_18": 0.4249099, "title+abstract_embedding_19": 0.23816898, "title+abstract_embedding_20": 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"title+abstract_embedding_111": -0.08621079, "title+abstract_embedding_112": -0.05778812, "title+abstract_embedding_113": -0.22724892, "title+abstract_embedding_114": -0.06304487, "title+abstract_embedding_115": 0.014572665, "title+abstract_embedding_116": 0.029429447, "title+abstract_embedding_117": 0.051223855, "title+abstract_embedding_118": -0.10278656, "title+abstract_embedding_119": 0.15293661, "title+abstract_embedding_120": -0.108480826, "title+abstract_embedding_121": -0.09192624, "title+abstract_embedding_122": 0.05359991, "title+abstract_embedding_123": -0.020749852, "title+abstract_embedding_124": -0.120454855, "title+abstract_embedding_125": -0.07594115, "title+abstract_embedding_126": 0.09667675, "title+abstract_embedding_127": -0.009215668, "label": 3, "label-multi": "3" }, { "paper_new_id": 18, "id": "j_16481873c250aeb29e1ef478c502f4dc", "title+abstract": "CoP3/CoMoP Heterogeneous Nanosheet Arrays as Robust Electrocatalyst for pH-Universal Hydrogen Evolution Reaction;Design and fabrication of a highly active and earth-abundant hydrogen evolution reaction (HER) electrocatalyst which can work in a wide range of pHs are pivotal for sustainable hydrogen production....", "title+abstract_embedding_0": -2.452993, "title+abstract_embedding_1": -0.47469983, "title+abstract_embedding_2": 0.2496973, "title+abstract_embedding_3": -0.7385187, "title+abstract_embedding_4": -0.36779863, "title+abstract_embedding_5": 0.029764116, "title+abstract_embedding_6": -0.024861783, "title+abstract_embedding_7": -0.2511268, "title+abstract_embedding_8": -0.44553113, "title+abstract_embedding_9": 0.6894502, "title+abstract_embedding_10": -0.4067672, "title+abstract_embedding_11": 0.7629547, "title+abstract_embedding_12": -0.27697745, "title+abstract_embedding_13": -0.21696573, "title+abstract_embedding_14": -0.35194704, "title+abstract_embedding_15": -0.29462722, "title+abstract_embedding_16": -0.019304037, "title+abstract_embedding_17": -0.48344696, 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0.14658295, "title+abstract_embedding_109": -0.10021723, "title+abstract_embedding_110": -0.08574167, "title+abstract_embedding_111": -0.06489019, "title+abstract_embedding_112": -0.041988954, "title+abstract_embedding_113": 0.007213578, "title+abstract_embedding_114": -0.1160218, "title+abstract_embedding_115": 0.047249366, "title+abstract_embedding_116": -0.05871828, "title+abstract_embedding_117": 0.049871776, "title+abstract_embedding_118": 0.08500839, "title+abstract_embedding_119": -0.057516985, "title+abstract_embedding_120": -0.055841047, "title+abstract_embedding_121": -0.14451736, "title+abstract_embedding_122": -0.20967314, "title+abstract_embedding_123": -0.07647267, "title+abstract_embedding_124": -0.17151022, "title+abstract_embedding_125": 0.004028171, "title+abstract_embedding_126": 0.081651405, "title+abstract_embedding_127": -0.012345672, "label": 3, "label-multi": "0;19;3" }, { "paper_new_id": 19, "id": "j_16c71bf999d8aa252bca3c20e97ba62c", "title+abstract": "Carbon nanotube reinforced nanocomposites for energy conversion and storage;Abstract CNT-reinforced foams comprised of three-dimensional (3D) interconnected macropores with uniform mesoporous walls were developed as multifunctional nanocomposites and tested for electrochemical energy conversion and storage. Multi-walled CNTs grown on the wall surface of the interconnected scaffold structure of carbon foams were found to improve the surface area and electrochemical properties of the nanocomposites. The lightweight CNT-reinforced nanocomposites not only exhibit high structural flexibility, but also possess enhanced electrocatalytic performance for HER at current density of 10?mA?cm?2 with overpotentials of 240?mV. In addition, these nanocomposites can be used as flexible, electric double layer capacitor electrodes, and have achieved a specific capacitance of 776?F?g?1, with excellent durability and stability after 1000 cycles.", "title+abstract_embedding_0": -0.59302145, "title+abstract_embedding_1": -1.1350127, "title+abstract_embedding_2": -1.3001748, "title+abstract_embedding_3": 0.5423012, "title+abstract_embedding_4": -0.3109663, "title+abstract_embedding_5": 0.7058602, "title+abstract_embedding_6": -0.3572195, "title+abstract_embedding_7": -0.15855019, "title+abstract_embedding_8": 0.42538458, "title+abstract_embedding_9": -0.15869427, "title+abstract_embedding_10": -0.2458141, "title+abstract_embedding_11": -0.6811049, "title+abstract_embedding_12": -0.89836836, "title+abstract_embedding_13": 0.1025084, "title+abstract_embedding_14": -0.10429597, "title+abstract_embedding_15": -0.003796697, "title+abstract_embedding_16": -0.105626985, "title+abstract_embedding_17": -0.037738338, 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and electrocatalytic properties of platinum on well-aligned carbon nanotube (CNT) arrays for methanol oxidation;Well-aligned carbon nanotube (CNT) arrays were used as supporting materials for platinum (Pt) electrocatalysts. The microstructure of the resulting Pt/aligned-CNT electrode was characterized by scanning electron microscopy (SEM), and nano-scale Pt catalysts dispersed highly on CNT arrays by electro-deposition can be obtained. The electrocatalytic properties of the Pt/aligned-CNT electrode for methanol oxidation have been investigated by cyclic voltammetry (CV). Compared with Pt/graphite and Pt/tangled-CNT/graphite electrodes, higher electrocatalytic activity of the Pt/aligned-CNT electrode can be observed. © 2005 Elsevier B.V.", "title+abstract_embedding_0": -0.94513136, "title+abstract_embedding_1": -0.75731945, "title+abstract_embedding_2": -1.3306808, "title+abstract_embedding_3": 0.6910571, "title+abstract_embedding_4": 0.52998847, "title+abstract_embedding_5": -0.09904081, "title+abstract_embedding_6": -0.19979677, "title+abstract_embedding_7": 0.26562437, "title+abstract_embedding_8": 0.6294979, "title+abstract_embedding_9": -0.889323, "title+abstract_embedding_10": 0.47640115, "title+abstract_embedding_11": -0.4020203, "title+abstract_embedding_12": 0.40139598, "title+abstract_embedding_13": -0.24787453, "title+abstract_embedding_14": -0.37015313, "title+abstract_embedding_15": 0.006761332, "title+abstract_embedding_16": 0.24873102, "title+abstract_embedding_17": 0.10734111, "title+abstract_embedding_18": 0.12736858, 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"title+abstract_embedding_109": -0.09490746, "title+abstract_embedding_110": -0.07819022, "title+abstract_embedding_111": -0.07764458, "title+abstract_embedding_112": -0.0678878, "title+abstract_embedding_113": -0.14187397, "title+abstract_embedding_114": 0.19913247, "title+abstract_embedding_115": -0.008071452, "title+abstract_embedding_116": 0.006170809, "title+abstract_embedding_117": -0.18692769, "title+abstract_embedding_118": 0.00279973, "title+abstract_embedding_119": 0.03218348, "title+abstract_embedding_120": 0.07892211, "title+abstract_embedding_121": -0.052571304, "title+abstract_embedding_122": -0.12988013, "title+abstract_embedding_123": 0.02131401, "title+abstract_embedding_124": 0.015055768, "title+abstract_embedding_125": 0.024596069, "title+abstract_embedding_126": 0.025565535, "title+abstract_embedding_127": -0.060755193, "label": 106, "label-multi": NaN }, { "paper_new_id": 21, "id": "j_18ce83444d4a8b29560660104415d40e", "title+abstract": "Highly efficient photocatalytic conversion of CO2 into solid CO using H2O as a reductant over Ag-modified ZnGa2O4;Highly crystalline ZnGa2O4 modified with Ag particles photocatalytically and selectively converted CO2 into CO (155.0 |¨¬mol h?1) using H2O as an electron donor.
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"title+abstract_embedding_114": 0.18991667, "title+abstract_embedding_115": -0.16587985, "title+abstract_embedding_116": 0.10965837, "title+abstract_embedding_117": 0.028981868, "title+abstract_embedding_118": -0.16080387, "title+abstract_embedding_119": -0.14275184, "title+abstract_embedding_120": 0.105509534, "title+abstract_embedding_121": 0.14713643, "title+abstract_embedding_122": 0.107831135, "title+abstract_embedding_123": 0.030457467, "title+abstract_embedding_124": -0.072662465, "title+abstract_embedding_125": 0.0959141, "title+abstract_embedding_126": -0.082377814, "title+abstract_embedding_127": 0.21865147, "label": 3, "label-multi": "1;17;3" }, { "paper_new_id": 22, "id": "j_1b70662660e2fa92006d534c869c08f7", "title+abstract": "Optimized Enhancement Effect of Sulfur in Fea??Na??S Codoped Carbon Nanosheets for Efficient Oxygen Reduction Reaction;The study on the design and preparation of oxygen reduction reaction (ORR) electrocatalysts with high efficiency is currently attracting great concern. Among different types of catalysts, heteroatom-doped carbon -based catalysts have exhibited promising potential, and the exploration of optimized matching of the doping elements is crucial to the design and fabrication of this category of catalysts. Herein, by annealing commercially available and costeffective precursors, Fe-N-S codoped graphene-like carbon nanosheet catalysts were prepared. The atomically dispersed Fe atoms coordinated with the N atoms to form FeN4 sites as proved by X-ray absorption spectroscopy. By facile modulation of the relative amount of the precursors, the contents of thiophene-S (Th-S) and Fe-N-4 sites could be tuned and a series of catalysts with different ThS/Fe ratios were prepared. The doped sulfur exhibited an enhancement effect on ORR performance, and strikingly, the enhancement efficiency could be optimized by fine modulation of the Th-S/Fe ratio in the catalysts. Furthermore, it was found that when the Th-S/Fe ratio reached an optimal value of 1.8, the ORR performance was significantly boosted, especially in acidic media. The experimental data were supported by density functional theory calculation results, which indicated that the ORR overpotential of the S-2(FeN4) configuration model (corresponding to the Th-S/Fe ratio of 2) was lower than that of S-3(FeN4) and S-1(FeN4). The optimized catalyst (denoted as FeN/SNC-900-3) displayed highly efficient ORR activity in both alkaline and acidic media. In alkaline media, the half-wave potential was 49 mV more positive than that of the commercial Pt/C catalyst, and in acidic media, the half-wave potential was close to that of Pt/C. Moreover, the stability of FeN/SNC-900-3 was outstanding, and the relative current density showed only a slight decay in both alkaline and acidic media after 40,000 s. A primary Zn air battery with FeN/SNC-900-3 as the cathode catalyst exhibited a high peak power density of up to 153 mW cm(-2) and superior cycling stability over 200 cycles.", "title+abstract_embedding_0": 0.5169233, "title+abstract_embedding_1": -0.76676244, "title+abstract_embedding_2": 0.36768332, "title+abstract_embedding_3": -0.9892436, "title+abstract_embedding_4": 0.69431704, "title+abstract_embedding_5": -0.22831053, "title+abstract_embedding_6": -0.07082611, "title+abstract_embedding_7": 0.11125513, "title+abstract_embedding_8": 0.2564727, "title+abstract_embedding_9": 0.011288703, "title+abstract_embedding_10": -0.24961816, "title+abstract_embedding_11": 0.39917397, "title+abstract_embedding_12": 0.50702953, "title+abstract_embedding_13": -0.065591015, "title+abstract_embedding_14": -0.07038331, "title+abstract_embedding_15": 0.16606045, "title+abstract_embedding_16": -0.010369599, "title+abstract_embedding_17": -0.0813048, "title+abstract_embedding_18": -0.14864247, "title+abstract_embedding_19": 0.34037128, "title+abstract_embedding_20": -0.20056486, "title+abstract_embedding_21": 0.36789125, "title+abstract_embedding_22": -0.21141014, "title+abstract_embedding_23": -0.16667564, "title+abstract_embedding_24": 0.031091928, "title+abstract_embedding_25": -0.2903511, "title+abstract_embedding_26": -0.12028064, "title+abstract_embedding_27": 0.09445215, "title+abstract_embedding_28": 0.14758077, "title+abstract_embedding_29": 0.24098073, "title+abstract_embedding_30": -0.12074056, "title+abstract_embedding_31": 0.10981513, "title+abstract_embedding_32": 0.24278307, "title+abstract_embedding_33": 0.15095657, "title+abstract_embedding_34": 0.24621335, "title+abstract_embedding_35": 0.12618917, "title+abstract_embedding_36": 0.1663999, "title+abstract_embedding_37": -0.3997681, "title+abstract_embedding_38": -0.050070487, "title+abstract_embedding_39": 0.05252076, "title+abstract_embedding_40": -0.22165805, "title+abstract_embedding_41": -0.17271762, 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"title+abstract_embedding_87": 0.18931513, "title+abstract_embedding_88": 0.07147446, "title+abstract_embedding_89": 0.009559505, "title+abstract_embedding_90": 0.008094996, "title+abstract_embedding_91": -0.021062955, "title+abstract_embedding_92": -0.08243565, "title+abstract_embedding_93": -0.021316592, "title+abstract_embedding_94": -0.051261075, "title+abstract_embedding_95": 0.13543604, "title+abstract_embedding_96": -0.10045216, "title+abstract_embedding_97": 0.010743767, "title+abstract_embedding_98": -0.12215111, "title+abstract_embedding_99": 0.12870443, "title+abstract_embedding_100": -0.012665764, "title+abstract_embedding_101": -0.052337725, "title+abstract_embedding_102": 0.09603442, "title+abstract_embedding_103": 0.08100289, "title+abstract_embedding_104": -0.18394232, "title+abstract_embedding_105": 0.087236, "title+abstract_embedding_106": -0.13520324, "title+abstract_embedding_107": -0.09252269, "title+abstract_embedding_108": -0.03693534, "title+abstract_embedding_109": 0.10459949, "title+abstract_embedding_110": -0.005305916, "title+abstract_embedding_111": 0.022068668, "title+abstract_embedding_112": 0.12626958, "title+abstract_embedding_113": -0.030494586, "title+abstract_embedding_114": -0.056865796, "title+abstract_embedding_115": -0.13912943, "title+abstract_embedding_116": 0.04532603, "title+abstract_embedding_117": -0.030226506, "title+abstract_embedding_118": 0.005843436, "title+abstract_embedding_119": 0.019973373, "title+abstract_embedding_120": 0.09895894, "title+abstract_embedding_121": 0.023049703, "title+abstract_embedding_122": -0.08882964, "title+abstract_embedding_123": 0.103678934, "title+abstract_embedding_124": 0.024448842, "title+abstract_embedding_125": 0.00169529, "title+abstract_embedding_126": 0.012858834, "title+abstract_embedding_127": 0.08366883, "label": 1, "label-multi": "1;15" }, { "paper_new_id": 23, "id": "j_1c06ba3019dbba92db809c3432bc2ebb", "title+abstract": "Characterization and photocatalytic activity of N-doped TiO2 prepared by thermal decomposition of Tia??melamine complex;Abstract Nitrogen doped spherical TiO 2 has been prepared by thermal decomposition of Ti¡§Cmelamine complex in air atmosphere. A clear shift in the onset light absorption from UV region ( 520?nm) has been observed for the N-doped samples. It has been deduced from the optical absorption spectra that the higher calcination temperature results in the decrease in the amount of N-doping. The XRD results revealed the phase transition of TiO 2 from anatase to rutile crystalline phase, starting at calcination temperature ?Y600???C. The electron microscopic images reveal the formation of spherical and flakes of TiO 2 nanocrystals (25?nm). The chemical nature of N in the N-TiO 2 has been evolved through X-ray photoelectron spectroscopy. The presence of different types of N species have been observed corresponding to different oxidation states and the presence of Ti¡§CN and O¡§CTi¡§CN have been confirmed from the observed binding energy values. Photocatalytic decomposition of methylene blue has been carried out both in the visible region and UV?+?visible region. In the visible region, N-TiO 2 showed higher activity compared to the undoped commercial TiO 2 (Degussa P25).", "title+abstract_embedding_0": 0.88145554, "title+abstract_embedding_1": 0.40239477, "title+abstract_embedding_2": 0.20582865, "title+abstract_embedding_3": 0.42778975, "title+abstract_embedding_4": 0.7256598, "title+abstract_embedding_5": -0.042890966, "title+abstract_embedding_6": 0.68513453, "title+abstract_embedding_7": 0.08870174, "title+abstract_embedding_8": -0.05450402, "title+abstract_embedding_9": 0.25938424, "title+abstract_embedding_10": 0.47545147, "title+abstract_embedding_11": -0.40764794, "title+abstract_embedding_12": -0.24236217, "title+abstract_embedding_13": 0.21194714, "title+abstract_embedding_14": 0.122419804, "title+abstract_embedding_15": 0.44649908, "title+abstract_embedding_16": 0.36798388, "title+abstract_embedding_17": 0.3908886, "title+abstract_embedding_18": 0.042937085, "title+abstract_embedding_19": 0.016945384, "title+abstract_embedding_20": 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"title+abstract_embedding_43": 0.07505493, "title+abstract_embedding_44": 0.10455944, "title+abstract_embedding_45": -0.09045714, "title+abstract_embedding_46": 0.006271303, "title+abstract_embedding_47": -0.025995038, "title+abstract_embedding_48": 0.03853698, "title+abstract_embedding_49": -0.1267977, "title+abstract_embedding_50": 0.122672915, "title+abstract_embedding_51": 0.0932042, "title+abstract_embedding_52": -0.07291944, "title+abstract_embedding_53": -0.019350074, "title+abstract_embedding_54": -0.001714632, "title+abstract_embedding_55": 0.30979055, "title+abstract_embedding_56": 0.085576326, "title+abstract_embedding_57": 0.20681739, "title+abstract_embedding_58": 0.002269477, "title+abstract_embedding_59": 0.00187999, "title+abstract_embedding_60": -0.000537038, "title+abstract_embedding_61": -0.027659185, "title+abstract_embedding_62": 0.3227375, "title+abstract_embedding_63": -0.1697104, "title+abstract_embedding_64": -0.023569405, "title+abstract_embedding_65": 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"title+abstract_embedding_88": 0.018850729, "title+abstract_embedding_89": -0.07182983, "title+abstract_embedding_90": -0.19615686, "title+abstract_embedding_91": -0.07670406, "title+abstract_embedding_92": -0.07754024, "title+abstract_embedding_93": -0.029451925, "title+abstract_embedding_94": 0.01956901, "title+abstract_embedding_95": 0.15452102, "title+abstract_embedding_96": 0.056455687, "title+abstract_embedding_97": 0.07383099, "title+abstract_embedding_98": -0.14698006, "title+abstract_embedding_99": 0.19990766, "title+abstract_embedding_100": 0.00914257, "title+abstract_embedding_101": 0.12282306, "title+abstract_embedding_102": 0.23892787, "title+abstract_embedding_103": -0.0474013, "title+abstract_embedding_104": 0.08128467, "title+abstract_embedding_105": -0.17860073, "title+abstract_embedding_106": 0.02779761, "title+abstract_embedding_107": -0.037246507, "title+abstract_embedding_108": -0.121399224, "title+abstract_embedding_109": 0.02957426, "title+abstract_embedding_110": -0.001839817, "title+abstract_embedding_111": -0.06321545, "title+abstract_embedding_112": 0.002825394, "title+abstract_embedding_113": -0.09257564, "title+abstract_embedding_114": 0.015259326, "title+abstract_embedding_115": 0.059297677, "title+abstract_embedding_116": 0.14157471, "title+abstract_embedding_117": -0.080754325, "title+abstract_embedding_118": 0.028557427, "title+abstract_embedding_119": -0.07382424, "title+abstract_embedding_120": 0.04763337, "title+abstract_embedding_121": 0.012310903, "title+abstract_embedding_122": -0.057330012, "title+abstract_embedding_123": -0.008116014, "title+abstract_embedding_124": 0.06373928, "title+abstract_embedding_125": 0.09742814, "title+abstract_embedding_126": -0.023949362, "title+abstract_embedding_127": 0.051107273, "label": 3, "label-multi": "0;3" }, { "paper_new_id": 24, "id": "j_1d06e503883ae12c7f3a6558de0adaa9", "title+abstract": "Plasma nitriding induced growth of Pt-nanowire arrays as high performance electrocatalysts for fuel cells;In this work, we demonstrate an innovative approach, combing a novel active screen plasma (ASP) technique with green chemical synthesis, for a direct fabrication of uniform Pt nanowire arrays on large-area supports. The ASP treatment enables in-situ N-doping and surface modification to the support surface, significantly promoting the uniform growth of tiny Pt nuclei which directs the growth of ultrathin single-crystal Pt nanowire (2.5¡§C3?nm in diameter) arrays, forming a three-dimensional (3D) nano-architecture. Pt nanowire arrays in-situ grown on the large-area gas diffusion layer (GDL) (5?cm2) can be directly used as the catalyst electrode in fuel cells. The unique design brings in an extremely thin electrocatalyst layer, facilitating the charge transfer and mass transfer properties, leading to over two times higher power density than the conventional Pt nanoparticle catalyst electrode in real fuel cell environment. Due to the similar challenges faced with other nanostructures and the high availability of ASP for other material surfaces, this work will provide valuable insights and guidance towards the development of other new nano-architectures for various practical applications.", "title+abstract_embedding_0": -0.46500558, "title+abstract_embedding_1": -0.8025583, "title+abstract_embedding_2": -1.2628607, "title+abstract_embedding_3": -0.022547364, "title+abstract_embedding_4": -0.16310596, "title+abstract_embedding_5": 0.7348962, "title+abstract_embedding_6": 0.019327134, "title+abstract_embedding_7": -0.26719895, "title+abstract_embedding_8": 0.1450861, "title+abstract_embedding_9": -0.26293212, "title+abstract_embedding_10": -0.3406524, "title+abstract_embedding_11": 0.22993106, "title+abstract_embedding_12": 0.55586934, "title+abstract_embedding_13": 0.012498416, "title+abstract_embedding_14": -0.34184536, "title+abstract_embedding_15": 0.67587227, "title+abstract_embedding_16": 0.24965954, 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"j_1daeddda48b718e2e486f67e18587db1", "title+abstract": "Synergetic Interaction of Additive Dual Nanocatalysts to Accelerate Oxygen Reduction Reaction in Fuel Cell Cathodes;The sluggish oxygen reduction reaction (ORR) in the cathode is hindering the power density of solid oxide fuel cells (SOFCs). Infiltration of catalyst into the cathode of SOFCs is promising to accelerate the ORR. However, the degradation associated with the coarsening of the nanocatalyst is intense. To stabilize the catalyst, atomic layer deposition (ALD) is employed to coat a dual electrocatalyst consisting of a superjacent 2 nm CoOx layer and superjacent 3 nm discrete Pt particles into the porous lanthanum strontium manganite (LSM)/yttria-stabilized zirconia (YSZ) cathode. After 504 h of operation at 750 ??C, the ALD coating resulted in the peak power density enhancement by ??200%, while CoOx becomes Mn-enriched (MnCo)Ox nanograins coupling with nano-Pt. The Pt/(MnCo)Ox nanocouplings are uniformly distributed on the YSZ grain surface, triple-phase boundaries, and at LSM/LSM surface grain boundaries. This study demonstrates an effective approach of stabilizing the minute amount of catalyst for enhancing OR...", "title+abstract_embedding_0": -0.10899639, "title+abstract_embedding_1": -0.9242779, "title+abstract_embedding_2": -0.3940744, "title+abstract_embedding_3": -0.824093, "title+abstract_embedding_4": 0.77573305, "title+abstract_embedding_5": -0.032003045, "title+abstract_embedding_6": -0.25421652, "title+abstract_embedding_7": 0.07147234, "title+abstract_embedding_8": 0.37805194, "title+abstract_embedding_9": -0.043900907, "title+abstract_embedding_10": -0.21591425, "title+abstract_embedding_11": 0.10726556, "title+abstract_embedding_12": 0.13290827, "title+abstract_embedding_13": 0.13678858, "title+abstract_embedding_14": -0.09643568, "title+abstract_embedding_15": 0.12999448, "title+abstract_embedding_16": 0.2909525, "title+abstract_embedding_17": -0.078009844, "title+abstract_embedding_18": 0.24898829, "title+abstract_embedding_19": 0.29663914, 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Performances and mechanisms;In this study, the adsorption and UV photocatalytic degradation of atrazine using nano-TiO2 particles were studied systematically, and the colloidal stability of nano-TiO2 particles in solution was also investigated to reveal the removal mechanism. Experiments which contained the first 6.0?hours darkness and 4.0?hours UV illumination later were conducted at different concentrations of Ca2+ and/or fulvic acids (FA) at pH?=?7.0. Results showed that the adsorption rate of atrazine onto nano-TiO2 particles decreased with the increase of Ca2+ and/or FA concentrations, which could be explained well by the colloidal stability of nanoparticles. When the solution contained Ca2+ or Ca2+-FA, the nanoparticles were aggregated together leading to the decrease of the contact surface area. Besides, there existed competitive adsorption between FA and atrazine on the particle surface. During photocatalytic degradation, the increase of Ca2+ and/or FA concentration accelerated the aggregation of nano-TiO2 particles and that reduced the degradation efficiency of atrazine. The particle sizes by SEM were in accordance with the aggregation degree of nanoparticles in the solutions. Sedimentation experiments of nano-TiO2 particles displayed that the fastest sedimentation was happened in the CaCl2 and FA coexistent system and followed by CaCl2 alone, and the results well demonstrated the photodegradation efficiency trends of atrazine by nano-TiO2 particles under the different sedimentation conditions.", "title+abstract_embedding_0": 1.1405951, "title+abstract_embedding_1": 0.30055338, "title+abstract_embedding_2": 0.12018204, "title+abstract_embedding_3": 0.7744235, "title+abstract_embedding_4": 0.37023836, "title+abstract_embedding_5": 0.21066171, "title+abstract_embedding_6": -0.2709417, "title+abstract_embedding_7": -0.17881063, "title+abstract_embedding_8": 0.039095387, "title+abstract_embedding_9": -0.3003165, "title+abstract_embedding_10": -0.33054435, "title+abstract_embedding_11": 0.042868637, "title+abstract_embedding_12": 0.06071797, "title+abstract_embedding_13": 0.23583204, "title+abstract_embedding_14": 0.08806515, "title+abstract_embedding_15": 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"label-multi": NaN }, { "paper_new_id": 27, "id": "j_1eaaff80f586afcf589419504023d26c", "title+abstract": "Plasmonic Titanium Nitride Facilitates Indium Oxide CO\n 2\n Photocatalysis;Nanoscale titanium nitride TiN is a metallic material that can effectively harvest sunlight over a broad spectral range and produce high local temperatures via the photothermal effect. Nanoscale indium oxide-hydroxide, In2O3-x(OH)(y), is a semiconducting material capable of photocatalyzing the hydrogenation of gaseous CO2; however, its wide electronic bandgap limits its absorption of photons to the ultraviolet region of the solar spectrum. Herein, the benefits of both nanomaterials in a ternary heterostructure: TiN@TiO2@In2O3-x(OH)(y) are combined. This heterostructured material synergistically couples the metallic TiN and semiconducting In2O3-x(OH)(y) phases via an interfacial semiconducting TiO2 layer, allowing it to drive the light-assisted reverse water gas shift reaction at a conversion rate greatly surpassing that of its individual components or any binary combinations thereof.", "title+abstract_embedding_0": -0.02507782, "title+abstract_embedding_1": 0.5010724, "title+abstract_embedding_2": -1.0156648, "title+abstract_embedding_3": 0.124361396, "title+abstract_embedding_4": 0.18168837, "title+abstract_embedding_5": 0.47826096, "title+abstract_embedding_6": 0.80735254, "title+abstract_embedding_7": -0.3277553, "title+abstract_embedding_8": -0.07131279, "title+abstract_embedding_9": -0.41297567, "title+abstract_embedding_10": -0.06847301, "title+abstract_embedding_11": -0.13472414, "title+abstract_embedding_12": 0.316702, "title+abstract_embedding_13": 0.70269185, "title+abstract_embedding_14": 0.12946892, 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"label-multi": "1;15;2;3" }, { "paper_new_id": 28, "id": "j_1f2ec268a44eabd814fe340db7659ca1", "title+abstract": "Reversing Interfacial Catalysis of Ambipolar WSe\n 2\n Single Crystal;An improved understanding of the origin of the electrocatalytic activity is of importance to the rational design of highly efficient electrocatalysts for the hydrogen evolution reaction. Here, an ambipolar single-crystal tungsten diselenide (WSe2) semiconductor is employed as a model system where the conductance and carrier of WSe2 can be individually tuned by external electric fields. The field-tuned electrochemical microcell is fabricated based on the single-crystal WSe2 and the catalytic activity of the WSe2 microcell is measured versus the external electric field. Results show that WSe2 with electrons serving as the dominant carrier yields much higher activity than WSe2 with holes serving as the dominant carrier even both systems exhibit similar conductance. The catalytic activity enhancement can be characterized by the Tafel slope decrease from 138 to 104 mV per decade, while the electron area concentration increases from 0.64 x 10(12) to 1.72 x 10(12) cm(-2). To further understand the underlying mechanism, the Gibbs free energy and charge distribution for adsorbed hydrogen on WSe2 versus the area charge concentration is systematically computed, which is in line with experiments. This comprehensive study not only sheds light on the mechanism underlying the electrocatalysis processes, but also offers a strategy to achieve higher electrocatalytic activity.", "title+abstract_embedding_0": 0.005898714, "title+abstract_embedding_1": -0.99222445, "title+abstract_embedding_2": 0.24103965, "title+abstract_embedding_3": -0.3294059, "title+abstract_embedding_4": 0.16317672, "title+abstract_embedding_5": 0.11658865, "title+abstract_embedding_6": 0.31703937, "title+abstract_embedding_7": -0.9121225, "title+abstract_embedding_8": -0.48610938, "title+abstract_embedding_9": 0.39043462, "title+abstract_embedding_10": 0.36504748, "title+abstract_embedding_11": 0.2679625, "title+abstract_embedding_12": 0.36524215, "title+abstract_embedding_13": -0.16973662, "title+abstract_embedding_14": 0.006534994, "title+abstract_embedding_15": -0.16882166, "title+abstract_embedding_16": 0.1987628, "title+abstract_embedding_17": -0.21921302, "title+abstract_embedding_18": -0.32295084, "title+abstract_embedding_19": -0.04071988, "title+abstract_embedding_20": 0.37331092, "title+abstract_embedding_21": -0.24824107, "title+abstract_embedding_22": -0.1337869, "title+abstract_embedding_23": -0.010585964, "title+abstract_embedding_24": -0.11828387, "title+abstract_embedding_25": 0.20955133, "title+abstract_embedding_26": -0.19166765, "title+abstract_embedding_27": 0.024183182, "title+abstract_embedding_28": -0.11919546, "title+abstract_embedding_29": 0.19482459, "title+abstract_embedding_30": 0.14060447, "title+abstract_embedding_31": 0.14463057, "title+abstract_embedding_32": -0.30344254, "title+abstract_embedding_33": 0.2848844, "title+abstract_embedding_34": -0.2015087, "title+abstract_embedding_35": 0.22688386, "title+abstract_embedding_36": -0.07191737, "title+abstract_embedding_37": 0.33613282, "title+abstract_embedding_38": -0.19929937, "title+abstract_embedding_39": 0.2699129, "title+abstract_embedding_40": -0.050376475, "title+abstract_embedding_41": 0.21019785, "title+abstract_embedding_42": -0.25061536, "title+abstract_embedding_43": -0.2130824, "title+abstract_embedding_44": 0.21378075, "title+abstract_embedding_45": 0.18891984, "title+abstract_embedding_46": 0.1798164, "title+abstract_embedding_47": -0.20090802, "title+abstract_embedding_48": 0.48491955, "title+abstract_embedding_49": 0.3411335, "title+abstract_embedding_50": -0.40119863, "title+abstract_embedding_51": -0.026939735, "title+abstract_embedding_52": -0.0760274, "title+abstract_embedding_53": -0.23183452, "title+abstract_embedding_54": 0.13163976, "title+abstract_embedding_55": 0.15205091, "title+abstract_embedding_56": 0.16114797, "title+abstract_embedding_57": -0.19894765, "title+abstract_embedding_58": -0.115805775, "title+abstract_embedding_59": -0.06185071, "title+abstract_embedding_60": -0.12069252, "title+abstract_embedding_61": -0.26617557, "title+abstract_embedding_62": -0.066316865, "title+abstract_embedding_63": -0.23805177, "title+abstract_embedding_64": -0.1049632, "title+abstract_embedding_65": 0.23880933, "title+abstract_embedding_66": 0.09737493, "title+abstract_embedding_67": 0.3364694, "title+abstract_embedding_68": 0.13828756, "title+abstract_embedding_69": -0.22878978, "title+abstract_embedding_70": 0.10784512, "title+abstract_embedding_71": -0.015486091, "title+abstract_embedding_72": 0.032206185, "title+abstract_embedding_73": -0.2522545, "title+abstract_embedding_74": -0.20372288, "title+abstract_embedding_75": -0.027609393, "title+abstract_embedding_76": 0.21906242, "title+abstract_embedding_77": 0.024553418, "title+abstract_embedding_78": 0.15883292, "title+abstract_embedding_79": -0.03360784, "title+abstract_embedding_80": 0.18957375, "title+abstract_embedding_81": 0.001609176, "title+abstract_embedding_82": 0.21513762, "title+abstract_embedding_83": 0.2007356, "title+abstract_embedding_84": -0.19315688, "title+abstract_embedding_85": -0.05321352, "title+abstract_embedding_86": -0.24023804, "title+abstract_embedding_87": -0.06895063, "title+abstract_embedding_88": -0.001605257, "title+abstract_embedding_89": 0.01512786, "title+abstract_embedding_90": -0.12446555, "title+abstract_embedding_91": -0.20754144, "title+abstract_embedding_92": -0.11187263, "title+abstract_embedding_93": 0.036708653, "title+abstract_embedding_94": -0.1307131, "title+abstract_embedding_95": 0.15295944, "title+abstract_embedding_96": -0.24371174, "title+abstract_embedding_97": -0.07643627, "title+abstract_embedding_98": 0.023098134, "title+abstract_embedding_99": -0.032076012, "title+abstract_embedding_100": 0.25008443, "title+abstract_embedding_101": 0.1236431, "title+abstract_embedding_102": -0.057693433, "title+abstract_embedding_103": -0.011848688, "title+abstract_embedding_104": 0.22535048, "title+abstract_embedding_105": -0.13446565, "title+abstract_embedding_106": -0.006830931, "title+abstract_embedding_107": -0.121283606, "title+abstract_embedding_108": 0.0809626, "title+abstract_embedding_109": 0.10386495, "title+abstract_embedding_110": 0.01802662, "title+abstract_embedding_111": -0.06803288, "title+abstract_embedding_112": 0.01051949, "title+abstract_embedding_113": 0.053491652, "title+abstract_embedding_114": 0.07965799, "title+abstract_embedding_115": -0.013311498, "title+abstract_embedding_116": 0.18088144, "title+abstract_embedding_117": 0.05963537, "title+abstract_embedding_118": -0.042470854, "title+abstract_embedding_119": -0.100427866, "title+abstract_embedding_120": 0.16734211, "title+abstract_embedding_121": -0.02263472, "title+abstract_embedding_122": -0.08802369, "title+abstract_embedding_123": 0.025984585, "title+abstract_embedding_124": -0.039979823, "title+abstract_embedding_125": -0.007715248, "title+abstract_embedding_126": -0.015783992, "title+abstract_embedding_127": -0.09170921, "label": 3, "label-multi": "1;15;3" }, { "paper_new_id": 29, "id": "j_232beae9d29cba84cf5b588285a1f36a", "title+abstract": "A novel poly(cyanocobalamin) modified glassy carbon electrode as electrochemical sensor for voltammetric determination of peroxynitrite;This report described the direct voltammetric detection of peroxynitrite (ONOO(-)) at a novel cyanocobalamin modified glassy carbon electrode prepared by electropolymeriation method. The electrochemical behaviors of peroxynitrite at the modified electrode were studied by cyclic voltammetry. The results showed that this new electrochemical sensor exhibited an excellent electrocatalytic activity to oxidation of peroxynitrite. The mechanism of catalysis was discussed. Based on electrocatalytic oxidation of peroxynitrite at the poly(cyanocobalamin) modified electrode, peroxynitrite was sensitively detected by differential pulse voltammetry. Under optimum conditions, the anodic peak current was linear to concentration of peroxynitrite in the range of 2.0 x 10(-6) to 3.0 x 10(-4) mol L(-1) with a detection limit of 1.0 x 10(-7) mol L(-1) (S/N of 3). The proposed method has been applied to determination of peroxynitrite in human serum with satisfactory results. This poly(cyanocobalamin) modified electrode showed high selectivity and sensitivity to peroxynitrite determination, which could be used in quantitative detection of peroxynitrite in vivo and in vitro. (C) 2010 Elsevier B.V. All rights reserved.", "title+abstract_embedding_0": 0.27821732, "title+abstract_embedding_1": -1.3187559, "title+abstract_embedding_2": 0.22866732, "title+abstract_embedding_3": 0.6313311, "title+abstract_embedding_4": -0.2790482, "title+abstract_embedding_5": -0.74714243, "title+abstract_embedding_6": -0.71429944, "title+abstract_embedding_7": 0.27927452, "title+abstract_embedding_8": -0.5631324, "title+abstract_embedding_9": -0.012194455, "title+abstract_embedding_10": 0.74626964, "title+abstract_embedding_11": -0.107056156, "title+abstract_embedding_12": -0.29101685, "title+abstract_embedding_13": -0.15020196, "title+abstract_embedding_14": -0.017239884, "title+abstract_embedding_15": -0.36827737, "title+abstract_embedding_16": 0.13851929, "title+abstract_embedding_17": 0.41972253, "title+abstract_embedding_18": -0.07999039, "title+abstract_embedding_19": -0.49653414, "title+abstract_embedding_20": -0.23005494, "title+abstract_embedding_21": 0.47317377, "title+abstract_embedding_22": 0.015408898, "title+abstract_embedding_23": -0.14696357, "title+abstract_embedding_24": -0.008450538, "title+abstract_embedding_25": 0.25798446, "title+abstract_embedding_26": 0.23874208, "title+abstract_embedding_27": 0.000273678, "title+abstract_embedding_28": -0.05053337, "title+abstract_embedding_29": -0.23151699, "title+abstract_embedding_30": -0.25035483, "title+abstract_embedding_31": 0.088901006, "title+abstract_embedding_32": -0.5715809, "title+abstract_embedding_33": -0.34602532, "title+abstract_embedding_34": 0.058373302, "title+abstract_embedding_35": -0.014272422, "title+abstract_embedding_36": -0.19104478, "title+abstract_embedding_37": 0.027671799, "title+abstract_embedding_38": 0.084466785, "title+abstract_embedding_39": -0.23526397, "title+abstract_embedding_40": 0.5223601, "title+abstract_embedding_41": -0.13589174, "title+abstract_embedding_42": -0.20287114, "title+abstract_embedding_43": 0.10738896, "title+abstract_embedding_44": -0.23530027, "title+abstract_embedding_45": 0.040960073, "title+abstract_embedding_46": -0.10568106, "title+abstract_embedding_47": 0.056547347, "title+abstract_embedding_48": 0.060937867, "title+abstract_embedding_49": -0.029031336, "title+abstract_embedding_50": 0.06005974, "title+abstract_embedding_51": -0.21766561, "title+abstract_embedding_52": -0.117917, "title+abstract_embedding_53": -0.23196101, "title+abstract_embedding_54": -0.28115875, "title+abstract_embedding_55": -0.02990907, "title+abstract_embedding_56": 0.0645027, "title+abstract_embedding_57": -0.11537685, "title+abstract_embedding_58": 0.075313404, "title+abstract_embedding_59": 0.014843807, "title+abstract_embedding_60": -0.033838928, "title+abstract_embedding_61": -0.11780331, "title+abstract_embedding_62": 0.06595045, "title+abstract_embedding_63": -0.1792551, "title+abstract_embedding_64": -0.05410269, "title+abstract_embedding_65": -0.020894557, "title+abstract_embedding_66": -0.001885023, "title+abstract_embedding_67": -0.13307698, "title+abstract_embedding_68": 0.27039814, "title+abstract_embedding_69": -0.08294767, "title+abstract_embedding_70": 0.004631996, "title+abstract_embedding_71": -0.021125734, "title+abstract_embedding_72": 0.14660147, "title+abstract_embedding_73": 0.088894434, "title+abstract_embedding_74": 0.33734792, "title+abstract_embedding_75": -0.1892615, "title+abstract_embedding_76": -0.088879675, "title+abstract_embedding_77": 0.15020546, "title+abstract_embedding_78": 0.046772838, "title+abstract_embedding_79": -0.16825226, "title+abstract_embedding_80": 0.025457263, "title+abstract_embedding_81": 0.093758345, "title+abstract_embedding_82": -0.16368943, "title+abstract_embedding_83": -0.12233266, "title+abstract_embedding_84": -0.052198067, "title+abstract_embedding_85": 0.11029595, "title+abstract_embedding_86": 0.14741926, "title+abstract_embedding_87": -0.0064684, "title+abstract_embedding_88": 0.012629166, "title+abstract_embedding_89": 0.10707144, "title+abstract_embedding_90": -0.015175976, "title+abstract_embedding_91": -0.17470455, "title+abstract_embedding_92": -0.122942284, "title+abstract_embedding_93": -0.11101204, "title+abstract_embedding_94": -0.15273255, "title+abstract_embedding_95": 0.06566533, "title+abstract_embedding_96": 0.034902364, "title+abstract_embedding_97": -0.20993884, "title+abstract_embedding_98": 0.102105364, "title+abstract_embedding_99": 0.14772034, "title+abstract_embedding_100": -0.105223194, "title+abstract_embedding_101": -0.09625845, "title+abstract_embedding_102": 0.01695989, "title+abstract_embedding_103": 0.19120914, "title+abstract_embedding_104": 0.028953, "title+abstract_embedding_105": -0.007747889, "title+abstract_embedding_106": 0.001489341, "title+abstract_embedding_107": -0.15789191, "title+abstract_embedding_108": -0.08688709, "title+abstract_embedding_109": 0.018774077, "title+abstract_embedding_110": -0.1251712, "title+abstract_embedding_111": -0.07643287, "title+abstract_embedding_112": -0.06610797, "title+abstract_embedding_113": -0.07099618, "title+abstract_embedding_114": -0.21826252, "title+abstract_embedding_115": -0.07433418, "title+abstract_embedding_116": 0.035916045, "title+abstract_embedding_117": -0.20730595, "title+abstract_embedding_118": 0.01733406, "title+abstract_embedding_119": 0.12048745, "title+abstract_embedding_120": 0.086114824, "title+abstract_embedding_121": 0.010438646, "title+abstract_embedding_122": 0.048986718, "title+abstract_embedding_123": -0.005435787, "title+abstract_embedding_124": 0.16686225, "title+abstract_embedding_125": -0.13604897, "title+abstract_embedding_126": 0.019045789, "title+abstract_embedding_127": 0.050857343, "label": 3, "label-multi": "3" }, { "paper_new_id": 30, "id": "j_23b6664067cf3bfeb5b342f28fbbb2e3", "title+abstract": "An overview of the methylene blue ISO test for assessing the activities of photocatalytic films;Abstract The main features are described of the ISO published standard: 10678:2010, namely the ??Determination of photocatalytic activity of surfaces in an aqueous medium by degradation of methylene blue?¡¥. The main underlying assumptions of the standard are considered, namely: (i) dye purity, (ii) adsorption and pH, (iii) light source, (iv) stirring and diffusion, (v) reaction mechanism and (vi) kinetics. Possible sources of errors arising form these assumptions are identified and changes to the standard's protocol suggested. The major suggested changes are: (i) a source of MB + of known and proven on site high purity (>90%) should be used to make up the standard test solution, which should have a referenced absorbance, 0.74, at 665?nm; (ii) the conditioning solution should be the same concentration as the standard test solution, (iii) the initial pH of the reaction solution should lie in the range: 5.5¡§C6.0; (iv) a BLB UVA light with a europium-doped strontium fluoroborate or borate phosphor should be used; (v) the reaction solution should be vigorously and continuously stirred if possible; (vi) the solution height should be the minimum recommended value of 2?cm, and the photoreactor cylinder i.d., 4.7?cm; (vii) after the 3?h irradiation the reaction solution should be left stirring overnight to check that no dye photoreductive bleaching has occurred. Application of most of these suggestions should improve considerably the standard's reported current poor percentage errors for repeatability within a lab (9.2%) and reproducibility between labs (30.6%).", "title+abstract_embedding_0": 0.6483462, "title+abstract_embedding_1": -0.37327477, "title+abstract_embedding_2": 1.2242433, "title+abstract_embedding_3": 0.3790154, "title+abstract_embedding_4": -0.52098405, "title+abstract_embedding_5": -0.13580197, "title+abstract_embedding_6": 0.3331866, "title+abstract_embedding_7": -0.005321093, "title+abstract_embedding_8": 0.2848827, "title+abstract_embedding_9": 0.025047094, "title+abstract_embedding_10": -0.2514941, "title+abstract_embedding_11": -0.40234256, "title+abstract_embedding_12": -0.00922218, "title+abstract_embedding_13": -0.24242166, "title+abstract_embedding_14": 0.18596649, "title+abstract_embedding_15": 0.4636417, "title+abstract_embedding_16": 0.30967814, "title+abstract_embedding_17": -0.008147702, "title+abstract_embedding_18": -0.32620934, "title+abstract_embedding_19": -0.1419668, "title+abstract_embedding_20": -0.036186397, "title+abstract_embedding_21": 0.19137996, "title+abstract_embedding_22": -0.2882738, "title+abstract_embedding_23": 0.042446136, "title+abstract_embedding_24": 0.039168373, "title+abstract_embedding_25": 0.064755976, "title+abstract_embedding_26": -0.24940717, "title+abstract_embedding_27": -0.25105137, "title+abstract_embedding_28": 0.24690187, "title+abstract_embedding_29": -0.0883982, "title+abstract_embedding_30": 0.13812283, "title+abstract_embedding_31": -0.5110126, "title+abstract_embedding_32": -0.021308482, "title+abstract_embedding_33": 0.116840854, "title+abstract_embedding_34": -0.26106733, "title+abstract_embedding_35": -0.08817552, "title+abstract_embedding_36": 0.17636359, "title+abstract_embedding_37": -0.12035239, "title+abstract_embedding_38": -0.046724338, "title+abstract_embedding_39": 0.23429295, "title+abstract_embedding_40": 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"title+abstract_embedding_63": -0.1756376, "title+abstract_embedding_64": -0.005008042, "title+abstract_embedding_65": 0.06639677, "title+abstract_embedding_66": -0.047699105, "title+abstract_embedding_67": 0.08794209, "title+abstract_embedding_68": 0.12246914, "title+abstract_embedding_69": -0.1844176, "title+abstract_embedding_70": -0.00565958, "title+abstract_embedding_71": -0.09972588, "title+abstract_embedding_72": 0.02675689, "title+abstract_embedding_73": 0.010166461, "title+abstract_embedding_74": 0.0672271, "title+abstract_embedding_75": -0.21027943, "title+abstract_embedding_76": -0.03606987, "title+abstract_embedding_77": 0.031081438, "title+abstract_embedding_78": 0.1342319, "title+abstract_embedding_79": -0.037583336, "title+abstract_embedding_80": -0.010374032, "title+abstract_embedding_81": -0.054663286, "title+abstract_embedding_82": -0.055357844, "title+abstract_embedding_83": -0.17292295, "title+abstract_embedding_84": 0.07463411, "title+abstract_embedding_85": 0.13009733, "title+abstract_embedding_86": 0.096618295, "title+abstract_embedding_87": 0.052933995, "title+abstract_embedding_88": 0.06908032, "title+abstract_embedding_89": 0.11307487, "title+abstract_embedding_90": 0.03627774, "title+abstract_embedding_91": 0.27059823, "title+abstract_embedding_92": 0.08795811, "title+abstract_embedding_93": -0.02245998, "title+abstract_embedding_94": -0.23446557, "title+abstract_embedding_95": -0.13547488, "title+abstract_embedding_96": 0.077324405, "title+abstract_embedding_97": 0.028189702, "title+abstract_embedding_98": -0.27142102, "title+abstract_embedding_99": -0.06872105, "title+abstract_embedding_100": -0.005749367, "title+abstract_embedding_101": 0.054797053, "title+abstract_embedding_102": -0.14493865, "title+abstract_embedding_103": -0.15754196, "title+abstract_embedding_104": 0.1098174, "title+abstract_embedding_105": -0.1457988, "title+abstract_embedding_106": -0.14813787, "title+abstract_embedding_107": 0.08042337, "title+abstract_embedding_108": 0.10871224, "title+abstract_embedding_109": -0.1876135, "title+abstract_embedding_110": 0.076370716, "title+abstract_embedding_111": -0.26430112, "title+abstract_embedding_112": 0.1261979, "title+abstract_embedding_113": 0.00706549, "title+abstract_embedding_114": -0.065491505, "title+abstract_embedding_115": -0.05550634, "title+abstract_embedding_116": 0.06428233, "title+abstract_embedding_117": -0.168312, "title+abstract_embedding_118": -0.07296697, "title+abstract_embedding_119": 0.068939045, "title+abstract_embedding_120": 0.096390456, "title+abstract_embedding_121": -0.052834027, "title+abstract_embedding_122": 0.103382796, "title+abstract_embedding_123": 0.069776766, "title+abstract_embedding_124": 0.119799264, "title+abstract_embedding_125": -0.002059542, "title+abstract_embedding_126": 0.075129226, "title+abstract_embedding_127": -0.0893143, "label": 3, "label-multi": "0;3" }, { "paper_new_id": 31, "id": "j_242b635a5143c8b318baf159c4f53f4e", "title+abstract": "Double-layer hybrid chainmail catalyst for high-performance hydrogen evolution;Developing highly catalytic active but stable MoS2 catalyst for electrochemical hydrogen evolution reaction (HER) performance, requires atomic-level tailoring of the electronic structure, but is greatly challenging. Herein, via precisely growing a double-layer MoS2/graphene hybrid structure encapsulating CoNi nanoalloy (MoS2/(CoNi@G)), we report both significantly enhanced HER activity and stability by the electrons of the CoNi cores traversing through the graphene to the outmost MoS2 layer. It achieves 10 mA cm(-2) at a significantly lower overpotential of 150 mV than that of 262 mV over pristine MoS2 nanosheets, and runs stably for over 10000 cyclic voltammetry cycles. The electron traversing effect efficiently tunes the electronic structures of both edge S sites and in-plane S vacancies, resulting in more appropriate adsorption energy of hydrogen on these active centers. It also induces strong electronic interactions between the MoS2 and CoNi@G, which stabilizes the outmost MoS2 layer and thereby significantly improves its catalytic stability.", "title+abstract_embedding_0": -0.3940708, "title+abstract_embedding_1": -0.8206991, "title+abstract_embedding_2": -0.35856274, "title+abstract_embedding_3": -0.9043187, "title+abstract_embedding_4": 0.6040103, "title+abstract_embedding_5": 0.19277868, "title+abstract_embedding_6": 0.2831091, "title+abstract_embedding_7": -0.66945016, "title+abstract_embedding_8": 0.1423024, "title+abstract_embedding_9": 0.58634853, "title+abstract_embedding_10": -0.037851937, "title+abstract_embedding_11": -0.24992718, "title+abstract_embedding_12": -0.023356915, "title+abstract_embedding_13": 0.23848656, "title+abstract_embedding_14": -0.108536765, "title+abstract_embedding_15": -0.19800822, "title+abstract_embedding_16": 0.23006308, "title+abstract_embedding_17": -0.57809186, "title+abstract_embedding_18": 0.2533092, "title+abstract_embedding_19": 0.21848592, "title+abstract_embedding_20": 0.079788, "title+abstract_embedding_21": 0.006432563, "title+abstract_embedding_22": 0.32391682, "title+abstract_embedding_23": 0.11976969, "title+abstract_embedding_24": -0.06863038, "title+abstract_embedding_25": 0.19427222, "title+abstract_embedding_26": -0.39004895, "title+abstract_embedding_27": -0.029055726, "title+abstract_embedding_28": -0.6528728, "title+abstract_embedding_29": -0.058980763, "title+abstract_embedding_30": 0.30542073, "title+abstract_embedding_31": 0.35201195, "title+abstract_embedding_32": 0.09952238, "title+abstract_embedding_33": 0.10736345, "title+abstract_embedding_34": -0.25104398, "title+abstract_embedding_35": 0.20345068, "title+abstract_embedding_36": 0.18740028, "title+abstract_embedding_37": -0.4193802, "title+abstract_embedding_38": 0.000205196, "title+abstract_embedding_39": 0.18366459, "title+abstract_embedding_40": 0.27505007, "title+abstract_embedding_41": 0.13678381, "title+abstract_embedding_42": -0.35083154, "title+abstract_embedding_43": 0.005919039, "title+abstract_embedding_44": -0.22401378, "title+abstract_embedding_45": 0.111404985, "title+abstract_embedding_46": -0.042576194, "title+abstract_embedding_47": 0.020628244, "title+abstract_embedding_48": 0.2225973, "title+abstract_embedding_49": 0.012284704, "title+abstract_embedding_50": 0.24300127, "title+abstract_embedding_51": 0.13868089, "title+abstract_embedding_52": -0.21913478, "title+abstract_embedding_53": 0.13900647, "title+abstract_embedding_54": -0.03006512, "title+abstract_embedding_55": -0.011649817, "title+abstract_embedding_56": 0.1405021, "title+abstract_embedding_57": -0.2505069, "title+abstract_embedding_58": 0.15617861, "title+abstract_embedding_59": 0.31340587, "title+abstract_embedding_60": 0.020652562, "title+abstract_embedding_61": -0.002428632, "title+abstract_embedding_62": 0.04887432, "title+abstract_embedding_63": 0.19169489, "title+abstract_embedding_64": 0.10755749, "title+abstract_embedding_65": -0.061745822, "title+abstract_embedding_66": 0.008183692, "title+abstract_embedding_67": 0.23311448, "title+abstract_embedding_68": -0.071964055, "title+abstract_embedding_69": -0.15423614, "title+abstract_embedding_70": -0.07610638, "title+abstract_embedding_71": 0.01883924, "title+abstract_embedding_72": 0.09570102, "title+abstract_embedding_73": -0.09478915, "title+abstract_embedding_74": -0.20047972, "title+abstract_embedding_75": -0.037092045, "title+abstract_embedding_76": -0.04408136, "title+abstract_embedding_77": -0.12599586, "title+abstract_embedding_78": 0.058682233, "title+abstract_embedding_79": -0.10914701, "title+abstract_embedding_80": -0.026658546, "title+abstract_embedding_81": -0.013222687, "title+abstract_embedding_82": 0.1567992, "title+abstract_embedding_83": 0.19971702, "title+abstract_embedding_84": 0.035295025, "title+abstract_embedding_85": -0.012363235, "title+abstract_embedding_86": -0.040696688, "title+abstract_embedding_87": 0.008802764, "title+abstract_embedding_88": 0.06819348, "title+abstract_embedding_89": 0.08331721, "title+abstract_embedding_90": -0.094758384, "title+abstract_embedding_91": -0.16428193, "title+abstract_embedding_92": 0.08793807, "title+abstract_embedding_93": 0.12394459, "title+abstract_embedding_94": 0.04206066, "title+abstract_embedding_95": 0.020290514, "title+abstract_embedding_96": -0.22196671, "title+abstract_embedding_97": -0.22168764, "title+abstract_embedding_98": -0.08085071, "title+abstract_embedding_99": 0.03932365, "title+abstract_embedding_100": 0.12798864, "title+abstract_embedding_101": -0.17188373, "title+abstract_embedding_102": 0.037152946, "title+abstract_embedding_103": 0.08712745, "title+abstract_embedding_104": -0.047676206, "title+abstract_embedding_105": -0.06902045, "title+abstract_embedding_106": -0.0819661, "title+abstract_embedding_107": -0.10420922, "title+abstract_embedding_108": 0.005466931, "title+abstract_embedding_109": 0.087675795, "title+abstract_embedding_110": -0.053706825, "title+abstract_embedding_111": 0.18682864, "title+abstract_embedding_112": -0.049156263, "title+abstract_embedding_113": 0.01876875, "title+abstract_embedding_114": -0.12411125, "title+abstract_embedding_115": 0.107576236, "title+abstract_embedding_116": -0.09199917, "title+abstract_embedding_117": 0.057648227, "title+abstract_embedding_118": -0.04987568, "title+abstract_embedding_119": -0.2213549, "title+abstract_embedding_120": -0.025374804, "title+abstract_embedding_121": 0.12703495, "title+abstract_embedding_122": 0.1532487, "title+abstract_embedding_123": -0.009789787, "title+abstract_embedding_124": 0.034289055, "title+abstract_embedding_125": 0.084990665, "title+abstract_embedding_126": 0.029649816, "title+abstract_embedding_127": 0.04332511, "label": 3, "label-multi": "1;15;2;3" }, { "paper_new_id": 32, "id": "j_253621b9c58e9eb6de26bfc559350a6d", "title+abstract": "Selective determination of dopamine in the presence of uric acid and ascorbic acid by N,Na?2-bis(indole-3-carboxaldimine)-1,2-diaminocyclohexane thin film modified glassy carbon electrode by differential pulse voltammetry;Abstract In this study N,N??-bis(indole-3-carboxaldimine)-1,2-diaminocyclohexane (ICDACH) was deposited on the glassy carbon (GC) electrode to fabricate a new sensor and used for the determination of dopamine. Deposition of ICDACH was performed by cyclic voltammetry scanning from 0.6?V to 1.7?V at a sweep rate of 100?mV?s ?1 for 25 cycles in 1?mM ICDACH solution. The prepared electrode was characterized by cyclic voltammetry (CV), electrochemical impedance spectroscopy (EIS), contact angle measurement (CAM), profilometry and X-ray photoelectron spectroscopy (XPS). The proposed electrode demonstrated an electrocatalytical effect on the oxidation of dopamine (DA) in the presence of 200?|¨¬M uric acid (UA) and 50?|¨¬M ascorbic acid (AA) using differential pulse voltammetry (DPV) method. The oxidation peak currents increased linearly with two concentration intervals of DA at pH 7 phosphate buffer. One of them is 0.60¡§C11.8?|¨¬M and the other is 11.8¡§C90.0?|¨¬M. The oxidation peaks of DA, UA and AA could be well separated because the oxidation of AA is inhibited on the modified electrode. Also the separation of DA and UA peak potentials are large enough for DA detection. Therefore, DA could be measured individually in the presence of UA and AA. The limit of detection (LOD) was found as 0.186?|¨¬M (at a signal-to-noise ratio of 3). The suggested electrode was applied for the determination of DA in dopamine hydrochloride injection and human urine sample with sufficient precision and accuracy.", "title+abstract_embedding_0": 0.71196353, "title+abstract_embedding_1": -1.0930122, "title+abstract_embedding_2": 0.7039671, "title+abstract_embedding_3": 0.25450385, "title+abstract_embedding_4": -0.28972566, "title+abstract_embedding_5": -0.7593076, "title+abstract_embedding_6": 0.075264126, "title+abstract_embedding_7": 0.47001395, "title+abstract_embedding_8": -0.46915814, "title+abstract_embedding_9": -0.5164932, "title+abstract_embedding_10": 0.3601426, "title+abstract_embedding_11": -0.10374371, "title+abstract_embedding_12": -0.35660473, "title+abstract_embedding_13": 0.07313951, "title+abstract_embedding_14": -0.18086253, "title+abstract_embedding_15": 0.06588737, "title+abstract_embedding_16": 0.4624151, "title+abstract_embedding_17": -0.107573345, "title+abstract_embedding_18": -0.047967046, "title+abstract_embedding_19": -0.19931646, "title+abstract_embedding_20": -0.34391487, "title+abstract_embedding_21": 0.48045418, "title+abstract_embedding_22": -0.52036744, "title+abstract_embedding_23": -0.32389447, "title+abstract_embedding_24": -0.024347827, "title+abstract_embedding_25": -0.35745996, "title+abstract_embedding_26": -0.066006586, "title+abstract_embedding_27": -0.4315294, "title+abstract_embedding_28": 0.29678616, "title+abstract_embedding_29": -0.40202436, "title+abstract_embedding_30": 0.10812557, "title+abstract_embedding_31": -0.04382363, "title+abstract_embedding_32": 0.23741153, "title+abstract_embedding_33": -0.18456492, "title+abstract_embedding_34": 0.08526297, "title+abstract_embedding_35": -0.15810195, "title+abstract_embedding_36": -0.35073045, "title+abstract_embedding_37": -0.11256416, "title+abstract_embedding_38": -0.008719437, "title+abstract_embedding_39": -0.072314255, "title+abstract_embedding_40": -0.06434104, "title+abstract_embedding_41": -0.22629575, "title+abstract_embedding_42": -0.2655656, "title+abstract_embedding_43": -0.0637254, "title+abstract_embedding_44": -0.1575505, "title+abstract_embedding_45": -0.030706167, "title+abstract_embedding_46": -0.031983316, "title+abstract_embedding_47": -0.076729834, "title+abstract_embedding_48": 0.07885361, "title+abstract_embedding_49": -0.077341475, "title+abstract_embedding_50": 0.1614787, "title+abstract_embedding_51": -0.105675906, "title+abstract_embedding_52": 0.002560884, "title+abstract_embedding_53": 0.19097514, "title+abstract_embedding_54": -0.16509762, "title+abstract_embedding_55": 0.25121593, "title+abstract_embedding_56": 0.152664, "title+abstract_embedding_57": 0.26430488, "title+abstract_embedding_58": -0.04853259, "title+abstract_embedding_59": 0.10125144, "title+abstract_embedding_60": -0.09472078, "title+abstract_embedding_61": -0.16018862, "title+abstract_embedding_62": -0.26659232, "title+abstract_embedding_63": 0.09233998, "title+abstract_embedding_64": -0.06891036, "title+abstract_embedding_65": -0.016075794, "title+abstract_embedding_66": -0.052372143, "title+abstract_embedding_67": -0.28183988, "title+abstract_embedding_68": 0.06162961, "title+abstract_embedding_69": -0.10857384, "title+abstract_embedding_70": 0.065489195, "title+abstract_embedding_71": -0.13427404, "title+abstract_embedding_72": 0.061049234, "title+abstract_embedding_73": -0.065761335, "title+abstract_embedding_74": 0.05246108, "title+abstract_embedding_75": 0.16964918, "title+abstract_embedding_76": -0.16165599, "title+abstract_embedding_77": 0.08952866, "title+abstract_embedding_78": 0.108872086, "title+abstract_embedding_79": -0.0584044, "title+abstract_embedding_80": 0.23246138, "title+abstract_embedding_81": 0.010387793, "title+abstract_embedding_82": 0.011321694, "title+abstract_embedding_83": 0.06391267, "title+abstract_embedding_84": 0.14977834, "title+abstract_embedding_85": -0.118635505, "title+abstract_embedding_86": -0.18834245, "title+abstract_embedding_87": 0.006658457, "title+abstract_embedding_88": 0.0217437, "title+abstract_embedding_89": -0.05437725, "title+abstract_embedding_90": 0.14000456, "title+abstract_embedding_91": -0.16722983, "title+abstract_embedding_92": 0.09316738, "title+abstract_embedding_93": -0.20275006, "title+abstract_embedding_94": 0.061865672, "title+abstract_embedding_95": -0.002718478, "title+abstract_embedding_96": 0.13530359, "title+abstract_embedding_97": 0.27516693, "title+abstract_embedding_98": 0.037259683, "title+abstract_embedding_99": -0.067409165, "title+abstract_embedding_100": -0.079643965, "title+abstract_embedding_101": -0.111500084, "title+abstract_embedding_102": 0.017443553, "title+abstract_embedding_103": 0.068382904, "title+abstract_embedding_104": -0.056566194, "title+abstract_embedding_105": 0.166301, "title+abstract_embedding_106": 0.12081845, "title+abstract_embedding_107": -0.065360054, "title+abstract_embedding_108": 0.03259719, "title+abstract_embedding_109": 0.008118197, "title+abstract_embedding_110": 0.13181037, "title+abstract_embedding_111": -0.09306201, "title+abstract_embedding_112": -0.08633666, "title+abstract_embedding_113": 0.024393767, "title+abstract_embedding_114": 0.14725369, "title+abstract_embedding_115": -0.025102608, "title+abstract_embedding_116": -0.10267384, "title+abstract_embedding_117": 0.12845112, "title+abstract_embedding_118": 0.1431748, "title+abstract_embedding_119": -0.13966075, "title+abstract_embedding_120": -0.014343778, "title+abstract_embedding_121": -0.06476668, "title+abstract_embedding_122": 0.013327271, "title+abstract_embedding_123": 0.023748048, "title+abstract_embedding_124": 0.02946917, "title+abstract_embedding_125": -0.036420308, "title+abstract_embedding_126": 0.09434688, "title+abstract_embedding_127": -0.06962636, "label": 3, "label-multi": "14;3" }, { "paper_new_id": 33, "id": "j_280bf3de25f57fba280bd74e1139e437", "title+abstract": "Novel PANI nanotube@TiO2 composite as efficient chemical and biological disinfectant;Abstract The objective of our study was to develop a new class of polyaniline/titanium dioxide (PANI¡§CTiO2) nanocomposites with characteristic one dimensional morphology. PANI¡§CTiO2 nanocomposites were characterized by SEM-EDX, TEM, UV¡§CDRS, TGA and XRD techniques. The PANI¡§CTiO2 nanocomposite was investigated for the photocatalysis and antibacterial properties; the latter was hitherto unscreened. The photocatalytic and antibacterial activity was tested using methylene blue (MB) as model dye and Escherichia coli (E. coli) as a model organism respectively. Antibacterial efficiency was analyzed by optical density and morphological damage was observed by TEM. In contrast to pristine polyaniline (PANI), lower concentrations of PANI¡§CTiO2 nanocomposite were needed to strongly inhibit the growth of wild-type E. coli. The nanocomposite has exceptionally good antibacterial activity against E. coli. Admirable photo-degradation efficiency against MB dye was achieved under visible light which could be attributed by the promotion of charge separation efficiency caused by the synergy between PANI and TiO2. Undoubtedly our results indicate that PANI¡§CTiO2 nanocomposite could be useful for multiple applications such as a very good candidate for water purification, antibiofouling, and disinfection of chemical and biological pollutants.", "title+abstract_embedding_0": 0.6145257, "title+abstract_embedding_1": 0.36364037, "title+abstract_embedding_2": -0.7448871, "title+abstract_embedding_3": 0.74735, "title+abstract_embedding_4": -0.4052708, "title+abstract_embedding_5": 0.3201993, "title+abstract_embedding_6": -0.65568423, "title+abstract_embedding_7": 0.1973897, "title+abstract_embedding_8": 0.16147527, "title+abstract_embedding_9": -0.14664584, "title+abstract_embedding_10": -0.046874017, "title+abstract_embedding_11": 0.03306642, "title+abstract_embedding_12": -0.068473876, "title+abstract_embedding_13": 0.48686257, "title+abstract_embedding_14": -0.13999647, "title+abstract_embedding_15": 0.32566866, "title+abstract_embedding_16": -0.39459002, "title+abstract_embedding_17": 0.336157, "title+abstract_embedding_18": -0.14812493, "title+abstract_embedding_19": 0.037358418, "title+abstract_embedding_20": -0.13631046, "title+abstract_embedding_21": -0.2779438, "title+abstract_embedding_22": 0.2299584, "title+abstract_embedding_23": 0.31487006, "title+abstract_embedding_24": -0.21307677, "title+abstract_embedding_25": 0.24979204, "title+abstract_embedding_26": -0.20114657, "title+abstract_embedding_27": 0.06878033, "title+abstract_embedding_28": -0.35260957, "title+abstract_embedding_29": 0.14069024, "title+abstract_embedding_30": 0.092187196, "title+abstract_embedding_31": 0.018502912, "title+abstract_embedding_32": -0.025050573, "title+abstract_embedding_33": 0.03768102, "title+abstract_embedding_34": -0.347437, "title+abstract_embedding_35": -0.091465205, "title+abstract_embedding_36": 0.35125932, "title+abstract_embedding_37": 0.21837671, "title+abstract_embedding_38": 0.25585708, "title+abstract_embedding_39": -0.013578491, "title+abstract_embedding_40": 0.16016862, "title+abstract_embedding_41": 0.23323044, "title+abstract_embedding_42": 0.3101419, "title+abstract_embedding_43": 0.114948854, "title+abstract_embedding_44": 0.21156307, "title+abstract_embedding_45": 0.22073841, "title+abstract_embedding_46": -0.06290144, "title+abstract_embedding_47": -0.33706668, "title+abstract_embedding_48": -0.16669257, "title+abstract_embedding_49": -0.15819444, "title+abstract_embedding_50": -0.09640172, "title+abstract_embedding_51": 0.19650374, "title+abstract_embedding_52": 0.20810686, "title+abstract_embedding_53": 0.03729562, "title+abstract_embedding_54": 0.09109883, "title+abstract_embedding_55": 0.06696599, "title+abstract_embedding_56": 0.16351216, "title+abstract_embedding_57": -0.27714044, "title+abstract_embedding_58": -0.054705665, "title+abstract_embedding_59": -0.20472057, "title+abstract_embedding_60": -0.014371723, "title+abstract_embedding_61": -0.18922856, "title+abstract_embedding_62": -0.06728245, "title+abstract_embedding_63": 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"title+abstract_embedding_108": 0.13561198, "title+abstract_embedding_109": 0.10693635, "title+abstract_embedding_110": -0.001932889, "title+abstract_embedding_111": 0.055798225, "title+abstract_embedding_112": -0.23226444, "title+abstract_embedding_113": 0.110063136, "title+abstract_embedding_114": 0.14158073, "title+abstract_embedding_115": -0.054847203, "title+abstract_embedding_116": 0.055815235, "title+abstract_embedding_117": 0.10029012, "title+abstract_embedding_118": -0.020248398, "title+abstract_embedding_119": 0.088504985, "title+abstract_embedding_120": -0.087111786, "title+abstract_embedding_121": 0.13199165, "title+abstract_embedding_122": 0.02161178, "title+abstract_embedding_123": 0.16375053, "title+abstract_embedding_124": 0.08870307, "title+abstract_embedding_125": 0.05533138, "title+abstract_embedding_126": -0.22429366, "title+abstract_embedding_127": 0.07359433, "label": 0, "label-multi": "0" }, { "paper_new_id": 34, "id": "j_280d7e0f1f6a59a436464f000f97ecbb", "title+abstract": "Photocatalytic Formation of Ia??I Bonds Using DNA Which Enables Detection of Single Nucleotide Polymorphisms;By decreasing the HOMO energy gap between the base-pairs to increase the charge conductivity of DNA, the positive charge photochemically generated in DNA can be made to migrate along the |D-way of DNA over long distances to form a long-lived charge-separated state. By fine-tuning the kinetics of the charge-transfer reactions, we designed a functionalized DNA system in which absorbed photon energy is converted into chemical energy to form I-I covalent bonds, where more than 100 I(2) molecules were produced per functionalized DNA. Utilizing the fact that charge-transfer kinetics through DNA is sensitive to the presence of a single mismatch that causes the perturbation of the |D-stacks, single nucleotide polymorphisms (SNPs) in genomic sequences were detected by measuring the photon energy conversion efficiency in DNA by a conventional starch iodine method.", "title+abstract_embedding_0": -0.4299904, "title+abstract_embedding_1": 0.044327438, "title+abstract_embedding_2": 0.5728818, "title+abstract_embedding_3": -0.3073063, "title+abstract_embedding_4": -0.7562241, "title+abstract_embedding_5": 0.4303234, "title+abstract_embedding_6": 0.30215454, "title+abstract_embedding_7": -0.33204278, "title+abstract_embedding_8": -0.28503472, "title+abstract_embedding_9": -0.50295866, "title+abstract_embedding_10": 0.26970074, "title+abstract_embedding_11": -0.0934557, "title+abstract_embedding_12": 0.13065101, "title+abstract_embedding_13": -0.085267045, "title+abstract_embedding_14": -0.122262344, 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"title+abstract_embedding_127": 0.12232757, "label": 3, "label-multi": "3" }, { "paper_new_id": 35, "id": "j_295b02f1c556a762b63a5c4246e18f32", "title+abstract": "Influence of Cr doping on the oxygen evolution potential of SnO2/Ti and Sb-SnO2/Ti electrodes;Oxygen evolution potential is the determining factor affecting the anode efficiency of the wastewater treatment process. In this study, we focus on increasing oxygen evolution potential of Cr-SnO2/Ti and Cr-Sb-SnO2/Ti electrodes with the pyrolytic method. XRD, SEM and XPS techniques had been applied to characterize the microstructures and chemical compositions of the samples. Electrochemical measurements had been performed to evaluate the oxygen evolution potential as a criterion of the wastewater treatment efficiency. The results show that co-doping of Sb and Cr improved the crystallinity and grain size of SnO2 coating, and Cr existed in the form of Cr(III) valence states. The Cr doping treatment improved the electronic conductivity and the electrocatalytic activity of the electrodes. DFT calculation of the band-structure indicates Cr doped SnO2 had a superior electrical conductivity, where Cr atom acts as an acceptor providing vacancies for electron transportation. The DOS diagrams reveal the Cr doped SnO2 showing a p-type conductivity which would subsequently influence the built-in potential on metal-semiconductor interface. We proposed the mechanism of the increase of oxygen evolution potential is the doping of Cr expands the built-in potential.", "title+abstract_embedding_0": 0.1323955, "title+abstract_embedding_1": -0.91559815, "title+abstract_embedding_2": 0.5419092, "title+abstract_embedding_3": 0.47972435, "title+abstract_embedding_4": 0.46363014, "title+abstract_embedding_5": -0.45101762, "title+abstract_embedding_6": 0.6241468, "title+abstract_embedding_7": -0.45903322, "title+abstract_embedding_8": -0.20275849, "title+abstract_embedding_9": 0.5010632, "title+abstract_embedding_10": 0.17826357, "title+abstract_embedding_11": 0.07550423, "title+abstract_embedding_12": 0.06132722, "title+abstract_embedding_13": -0.0857957, "title+abstract_embedding_14": 0.09343523, "title+abstract_embedding_15": -0.24884787, "title+abstract_embedding_16": -0.27901298, "title+abstract_embedding_17": -0.19568564, "title+abstract_embedding_18": 0.10441083, "title+abstract_embedding_19": 0.037773006, "title+abstract_embedding_20": -0.115236014, "title+abstract_embedding_21": -0.41115934, "title+abstract_embedding_22": -0.23470429, "title+abstract_embedding_23": -0.019760877, "title+abstract_embedding_24": 0.005582258, "title+abstract_embedding_25": 0.08087087, "title+abstract_embedding_26": 0.23739746, "title+abstract_embedding_27": 0.07995784, "title+abstract_embedding_28": -0.043387175, "title+abstract_embedding_29": 0.32074663, "title+abstract_embedding_30": 0.13929021, "title+abstract_embedding_31": -0.13141122, "title+abstract_embedding_32": 0.3622317, "title+abstract_embedding_33": 0.098058164, "title+abstract_embedding_34": -0.48914453, "title+abstract_embedding_35": -0.050326817, "title+abstract_embedding_36": 0.087432176, "title+abstract_embedding_37": -0.17215246, "title+abstract_embedding_38": 0.17754835, "title+abstract_embedding_39": 0.2671938, "title+abstract_embedding_40": 0.008865893, "title+abstract_embedding_41": -0.11982176, "title+abstract_embedding_42": 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"title+abstract_embedding_65": 0.19888304, "title+abstract_embedding_66": 0.094847575, "title+abstract_embedding_67": 0.20036945, "title+abstract_embedding_68": -0.13173187, "title+abstract_embedding_69": 0.10995899, "title+abstract_embedding_70": 0.16083011, "title+abstract_embedding_71": 0.03596881, "title+abstract_embedding_72": -0.018409908, "title+abstract_embedding_73": 0.027624905, "title+abstract_embedding_74": 0.19592074, "title+abstract_embedding_75": 0.08446738, "title+abstract_embedding_76": -0.2604691, "title+abstract_embedding_77": 0.088999406, "title+abstract_embedding_78": 0.33207065, "title+abstract_embedding_79": 0.17595564, "title+abstract_embedding_80": 0.28471833, "title+abstract_embedding_81": 0.06181979, "title+abstract_embedding_82": 0.14419034, "title+abstract_embedding_83": -0.15611131, "title+abstract_embedding_84": -0.117145106, "title+abstract_embedding_85": -0.10708618, "title+abstract_embedding_86": 0.071846545, "title+abstract_embedding_87": 0.12598723, 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-0.027268603, "title+abstract_embedding_111": 0.11060039, "title+abstract_embedding_112": 0.108687036, "title+abstract_embedding_113": -0.097356364, "title+abstract_embedding_114": -0.018431291, "title+abstract_embedding_115": -0.057927333, "title+abstract_embedding_116": 0.11452636, "title+abstract_embedding_117": -0.097672865, "title+abstract_embedding_118": -0.078905456, "title+abstract_embedding_119": 0.00585906, "title+abstract_embedding_120": -0.07380882, "title+abstract_embedding_121": 0.1562426, "title+abstract_embedding_122": -0.13230357, "title+abstract_embedding_123": 0.12249627, "title+abstract_embedding_124": -0.049037628, "title+abstract_embedding_125": 0.057308163, "title+abstract_embedding_126": 0.10428296, "title+abstract_embedding_127": -0.10178521, "label": 3, "label-multi": "14;3" }, { "paper_new_id": 36, "id": "j_2bc357a96044600c58c6998959d2795f", "title+abstract": "Seamlessly Splicing Metallic Sn\n \n x\n \n Mo\n 1a??\n \n x\n \n S\n 2\n at MoS\n 2\n Edge for Enhanced Photoelectrocatalytic Performance in Microreactor;Accurate design of the 2D metal-semiconductor (M-S) heterostructure via the covalent combination of appropriate metallic and semiconducting materials is urgently needed for fabricating high-performance nanodevices and enhancing catalytic performance. Hence, the lateral epitaxial growth of M-S SnxMo1-xS2/MoS2 heterostructure is precisely prepared with in situ growth of metallic SnxMo1-xS2 by doping Sn atoms at semiconductor MoS2 edge via one-step chemical vapor deposition. The atomically sharp interface of this heterostructure exhibits clearly distinguished performance based on a series of characterizations. The oxygen evolution photoelectrocatalytic performance of the epitaxial M-S heterostructure is 2.5 times higher than that of pure MoS2 in microreactor, attributed to the efficient electron-hole separation and rapid charge transfer. This growth method provides a general strategy for fabricating seamless M-S lateral heterostructures by controllable doping heteroatoms. The M-S heterostructures show increased carrier migration rate and eliminated Fermi level pinning effect, contributing to their potential in devices and catalytic system.", "title+abstract_embedding_0": 0.48688138, "title+abstract_embedding_1": -0.13874759, "title+abstract_embedding_2": -0.5886239, "title+abstract_embedding_3": -1.0150411, "title+abstract_embedding_4": -0.023817837, "title+abstract_embedding_5": 0.1860444, "title+abstract_embedding_6": 0.45337072, "title+abstract_embedding_7": -0.100964755, "title+abstract_embedding_8": -0.42927033, "title+abstract_embedding_9": 0.24693161, "title+abstract_embedding_10": -0.15757962, "title+abstract_embedding_11": -0.09163606, "title+abstract_embedding_12": 0.33659664, "title+abstract_embedding_13": 0.38450712, "title+abstract_embedding_14": 0.18832669, "title+abstract_embedding_15": -0.08901673, "title+abstract_embedding_16": 0.089850485, "title+abstract_embedding_17": -0.0804124, "title+abstract_embedding_18": -0.15555014, 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"title+abstract_embedding_87": -0.18342789, "title+abstract_embedding_88": -0.08727639, "title+abstract_embedding_89": 0.04637948, "title+abstract_embedding_90": 0.06449042, "title+abstract_embedding_91": -0.04362198, "title+abstract_embedding_92": -0.19034564, "title+abstract_embedding_93": 0.08922023, "title+abstract_embedding_94": 0.09809689, "title+abstract_embedding_95": 0.11014702, "title+abstract_embedding_96": -0.11236676, "title+abstract_embedding_97": -0.27645293, "title+abstract_embedding_98": 0.06486059, "title+abstract_embedding_99": -0.14160681, "title+abstract_embedding_100": 0.13721046, "title+abstract_embedding_101": -0.22644532, "title+abstract_embedding_102": 0.21689197, "title+abstract_embedding_103": -0.021523282, "title+abstract_embedding_104": 0.10681427, "title+abstract_embedding_105": 0.17148069, "title+abstract_embedding_106": -0.11751443, "title+abstract_embedding_107": 0.11326863, "title+abstract_embedding_108": -0.1947434, "title+abstract_embedding_109": 0.013600066, "title+abstract_embedding_110": -0.23830265, "title+abstract_embedding_111": 0.2910341, "title+abstract_embedding_112": 0.001074433, "title+abstract_embedding_113": 0.18775901, "title+abstract_embedding_114": 0.043941274, "title+abstract_embedding_115": 0.02724725, "title+abstract_embedding_116": 0.014791265, "title+abstract_embedding_117": -0.05042319, "title+abstract_embedding_118": 0.006923537, "title+abstract_embedding_119": -0.009628367, "title+abstract_embedding_120": -0.017568221, "title+abstract_embedding_121": 0.070432834, "title+abstract_embedding_122": -0.034211785, "title+abstract_embedding_123": 0.14887634, "title+abstract_embedding_124": -0.065456204, "title+abstract_embedding_125": -0.026477009, "title+abstract_embedding_126": 0.09732303, "title+abstract_embedding_127": -0.05258286, "label": 3, "label-multi": "1;15;3" }, { "paper_new_id": 37, "id": "j_2cad82bd352e9538516d61a958dc66ce", "title+abstract": "Single-Metal Atom Anchored on Boron Monolayer (?212) as an Electrocatalyst for Nitrogen Reduction into Ammonia at Ambient Conditions: A First-Principles Study;On the basis of the first-principles calculation, single transition-metal (TM) atoms of first and second transition series are anchored on the phase of the boron monolayer (BM) electrocatalyst for the sustainable production of ammonia (NH3) by reducing nitrogen (N-2). We have found a new type of electrocatalyst, i.e., V atom support on the beta(12)-BM (V/beta(12)-BM), which has a low onset potential (0.28 V), low cost, high stability, high selectivity, and high efficiency under mild conditions. The difference charge density and local density of state further demonstrated that there is an \"acceptance-donation\" interaction between TM atom and N-2, and the ionization of In orbital of N-2 can greatly elongate the N-N bond length, leading to the activity enhancement of N-2. We also point out that the bonding orbital (1 pi) and antibonding orbital (1 pi*) of N-2 play a crucial role in increasing the activity of N-2. Further, the climbing nudged elastic band method and molecular dynamics simulation indicate that V/beta(12)-BM has high dynamic and thermodynamic stabilities. Moreover, V/beta(12)-BM can also effectively suppress the hydrogen evolution reaction during the whole N-2 reduction reaction process. So, we propose V/beta(12)-BM as an excellent and promising catalyst for N-2 reduction to NH3 at ambient conditions.", "title+abstract_embedding_0": 0.21123827, "title+abstract_embedding_1": -0.9190999, "title+abstract_embedding_2": 0.34517854, "title+abstract_embedding_3": -0.6267718, "title+abstract_embedding_4": 0.28110093, "title+abstract_embedding_5": 0.33162254, "title+abstract_embedding_6": 0.39195514, "title+abstract_embedding_7": 0.036191754, "title+abstract_embedding_8": -0.18125623, "title+abstract_embedding_9": 0.044187516, "title+abstract_embedding_10": -0.4057494, "title+abstract_embedding_11": -0.22986943, "title+abstract_embedding_12": 0.4386922, "title+abstract_embedding_13": 0.010919455, "title+abstract_embedding_14": 0.059675574, "title+abstract_embedding_15": 0.16101393, "title+abstract_embedding_16": -0.2599882, "title+abstract_embedding_17": -0.075195804, "title+abstract_embedding_18": 0.10312171, "title+abstract_embedding_19": -0.101150945, "title+abstract_embedding_20": -0.007202849, "title+abstract_embedding_21": -0.18597116, "title+abstract_embedding_22": -0.3549686, "title+abstract_embedding_23": 0.019592643, "title+abstract_embedding_24": -0.041172594, "title+abstract_embedding_25": 0.11534512, "title+abstract_embedding_26": -0.14467967, "title+abstract_embedding_27": 0.09905559, "title+abstract_embedding_28": 0.29226172, "title+abstract_embedding_29": 0.06866002, "title+abstract_embedding_30": 0.17193165, "title+abstract_embedding_31": -0.22140008, "title+abstract_embedding_32": 0.0514239, "title+abstract_embedding_33": 0.29227397, "title+abstract_embedding_34": -0.12841988, "title+abstract_embedding_35": -0.29719266, "title+abstract_embedding_36": 0.3023366, "title+abstract_embedding_37": 0.031245768, "title+abstract_embedding_38": -0.002803586, "title+abstract_embedding_39": -0.2104308, "title+abstract_embedding_40": 0.101133615, "title+abstract_embedding_41": 0.07548795, "title+abstract_embedding_42": 0.15114507, "title+abstract_embedding_43": 0.100831285, "title+abstract_embedding_44": -0.018162817, "title+abstract_embedding_45": 0.12529129, "title+abstract_embedding_46": 0.31003824, "title+abstract_embedding_47": 0.11655508, "title+abstract_embedding_48": -0.009853348, "title+abstract_embedding_49": 0.1857166, "title+abstract_embedding_50": -0.05360186, "title+abstract_embedding_51": 0.04732342, "title+abstract_embedding_52": 0.18827383, "title+abstract_embedding_53": 0.18733421, "title+abstract_embedding_54": 0.082763895, "title+abstract_embedding_55": -0.15523657, "title+abstract_embedding_56": 0.05883413, "title+abstract_embedding_57": 0.25332245, "title+abstract_embedding_58": -0.011203364, "title+abstract_embedding_59": 0.032087862, "title+abstract_embedding_60": -0.092040956, "title+abstract_embedding_61": 0.086279385, "title+abstract_embedding_62": -0.04869456, "title+abstract_embedding_63": 0.06765919, "title+abstract_embedding_64": -0.23817538, "title+abstract_embedding_65": 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"title+abstract_embedding_88": -0.001322314, "title+abstract_embedding_89": 0.16023463, "title+abstract_embedding_90": 0.16446796, "title+abstract_embedding_91": 0.23003644, "title+abstract_embedding_92": 0.051617205, "title+abstract_embedding_93": -0.102981836, "title+abstract_embedding_94": -0.012840189, "title+abstract_embedding_95": -0.013279714, "title+abstract_embedding_96": -0.16493985, "title+abstract_embedding_97": -0.012304792, "title+abstract_embedding_98": -0.06041791, "title+abstract_embedding_99": 0.03888087, "title+abstract_embedding_100": -0.00557065, "title+abstract_embedding_101": -0.30208406, "title+abstract_embedding_102": -0.008417118, "title+abstract_embedding_103": 0.060960695, "title+abstract_embedding_104": 0.046584398, "title+abstract_embedding_105": -0.15110184, "title+abstract_embedding_106": -0.031636238, "title+abstract_embedding_107": 0.0509926, "title+abstract_embedding_108": -0.03227295, "title+abstract_embedding_109": -0.025689662, "title+abstract_embedding_110": 0.17537194, "title+abstract_embedding_111": -0.135425, "title+abstract_embedding_112": -0.08827247, "title+abstract_embedding_113": -0.14868908, "title+abstract_embedding_114": 0.038503602, "title+abstract_embedding_115": 0.05005313, "title+abstract_embedding_116": 0.10230076, "title+abstract_embedding_117": -0.12281294, "title+abstract_embedding_118": -0.055201203, "title+abstract_embedding_119": -0.08080006, "title+abstract_embedding_120": 0.008108709, "title+abstract_embedding_121": 0.070580296, "title+abstract_embedding_122": -0.1210649, "title+abstract_embedding_123": 0.018020757, "title+abstract_embedding_124": -0.038378708, "title+abstract_embedding_125": -0.022836067, "title+abstract_embedding_126": -0.029450234, "title+abstract_embedding_127": -0.08401632, "label": 3, "label-multi": "1;15;3" }, { "paper_new_id": 38, "id": "j_2e913ca15e1e3599ed8b685d04543048", "title+abstract": "Electrocatalysis for Chlorine Electrode Reaction on RuO2 Electrode in NaAlCl4 Melt;In molten with near equimolar compositions, electrocatalysis of the chlorine electrode reaction on electrodes has been investigated at 175??C. Melt?\\stable electrodes were prepared by a thermal decomposition method on semiconductive films deposited on Pyrex substrates. Tafel relationships for chlorine evolution and reduction were studied as functions of and partial pressure of , and several kinetic parameters including reaction orders with respect to Cl? and were determined. The mechanistic analysis based on the theoretical kinetic derivatives revealed that the chlorine electrode reaction on obeys a Volmer?\\Tafel type mechanism under the activated Temkin condition: (fast), (slow). The exchange current density at the standard condition (, ) was , and this figure was found to be 15¡§C20 times larger than that on glassy carbon electrodes. The difference of this electrocatalytic activity was ascribed to the mechanistic difference between the two electrode materials and not to the difference of electrode roughness. Capacity data to check this viewpoint were also presented.", "title+abstract_embedding_0": -0.255082, "title+abstract_embedding_1": -0.82183516, "title+abstract_embedding_2": 0.7387196, "title+abstract_embedding_3": 0.65076417, "title+abstract_embedding_4": 0.2995034, "title+abstract_embedding_5": -0.095651925, "title+abstract_embedding_6": 0.57184595, "title+abstract_embedding_7": -0.120440066, "title+abstract_embedding_8": -0.3062936, "title+abstract_embedding_9": 0.08973342, "title+abstract_embedding_10": 0.33020753, "title+abstract_embedding_11": -0.14571205, "title+abstract_embedding_12": -0.09743872, "title+abstract_embedding_13": -0.46888766, "title+abstract_embedding_14": 0.113396436, "title+abstract_embedding_15": 0.10315996, "title+abstract_embedding_16": 0.34628773, "title+abstract_embedding_17": -0.113550454, "title+abstract_embedding_18": -0.40421313, "title+abstract_embedding_19": 0.002465132, "title+abstract_embedding_20": 0.116016194, "title+abstract_embedding_21": 0.11757219, "title+abstract_embedding_22": 0.14334533, "title+abstract_embedding_23": 0.20508623, "title+abstract_embedding_24": -0.32924083, "title+abstract_embedding_25": -0.04968047, "title+abstract_embedding_26": 0.2123256, "title+abstract_embedding_27": -0.09966652, "title+abstract_embedding_28": -0.30716962, "title+abstract_embedding_29": 0.21753941, "title+abstract_embedding_30": 0.49692395, "title+abstract_embedding_31": 0.09579657, "title+abstract_embedding_32": 0.2593801, "title+abstract_embedding_33": -0.22886673, "title+abstract_embedding_34": -0.18049127, "title+abstract_embedding_35": 0.09665022, "title+abstract_embedding_36": 0.18030617, "title+abstract_embedding_37": 0.1782438, "title+abstract_embedding_38": 0.018849574, "title+abstract_embedding_39": -0.11106727, "title+abstract_embedding_40": -7.34e-05, "title+abstract_embedding_41": -0.025523499, "title+abstract_embedding_42": -0.06620577, "title+abstract_embedding_43": 0.29346788, "title+abstract_embedding_44": -0.337815, "title+abstract_embedding_45": -0.31401163, "title+abstract_embedding_46": 0.09574473, "title+abstract_embedding_47": -0.20772974, "title+abstract_embedding_48": 0.08733511, "title+abstract_embedding_49": 0.17822963, "title+abstract_embedding_50": 0.06047737, "title+abstract_embedding_51": -0.084612876, "title+abstract_embedding_52": -0.18302694, "title+abstract_embedding_53": 0.009798504, "title+abstract_embedding_54": -0.16077732, "title+abstract_embedding_55": 0.14516413, "title+abstract_embedding_56": -0.13101566, "title+abstract_embedding_57": -0.14904407, "title+abstract_embedding_58": -0.04904802, "title+abstract_embedding_59": -0.17602004, "title+abstract_embedding_60": 0.09322342, "title+abstract_embedding_61": 0.09069319, "title+abstract_embedding_62": -0.14230022, "title+abstract_embedding_63": -0.061406113, "title+abstract_embedding_64": 0.09374304, "title+abstract_embedding_65": -0.17799392, "title+abstract_embedding_66": 0.047915537, "title+abstract_embedding_67": 0.0677093, "title+abstract_embedding_68": -0.22126663, "title+abstract_embedding_69": 0.08810052, "title+abstract_embedding_70": 0.1907506, "title+abstract_embedding_71": 0.1760229, "title+abstract_embedding_72": 0.3808071, "title+abstract_embedding_73": -0.1890519, "title+abstract_embedding_74": -0.022182543, "title+abstract_embedding_75": -0.18809018, "title+abstract_embedding_76": -0.000974178, "title+abstract_embedding_77": -0.09307368, "title+abstract_embedding_78": 0.1822428, "title+abstract_embedding_79": -0.03291619, "title+abstract_embedding_80": -0.035617497, "title+abstract_embedding_81": 0.08461272, "title+abstract_embedding_82": 0.14549221, "title+abstract_embedding_83": -0.1868439, "title+abstract_embedding_84": 0.2139697, "title+abstract_embedding_85": -0.07081951, "title+abstract_embedding_86": -0.088606425, "title+abstract_embedding_87": 0.10488257, "title+abstract_embedding_88": -0.053495973, "title+abstract_embedding_89": 0.093020335, "title+abstract_embedding_90": 0.18481947, "title+abstract_embedding_91": 0.08219975, "title+abstract_embedding_92": -0.19469348, "title+abstract_embedding_93": 0.05968953, "title+abstract_embedding_94": -0.011130251, "title+abstract_embedding_95": -0.040917978, "title+abstract_embedding_96": 0.11202105, "title+abstract_embedding_97": -0.07742158, "title+abstract_embedding_98": -0.10325332, "title+abstract_embedding_99": 0.1016219, "title+abstract_embedding_100": 0.07881509, "title+abstract_embedding_101": -0.009728566, "title+abstract_embedding_102": -0.02805315, "title+abstract_embedding_103": -0.025529668, "title+abstract_embedding_104": 0.094754346, "title+abstract_embedding_105": 0.118738115, "title+abstract_embedding_106": 0.21580389, "title+abstract_embedding_107": 0.017768962, "title+abstract_embedding_108": -0.010204125, "title+abstract_embedding_109": 0.009322137, "title+abstract_embedding_110": 0.11478257, "title+abstract_embedding_111": -0.1422672, "title+abstract_embedding_112": -0.017580673, "title+abstract_embedding_113": 0.030260585, "title+abstract_embedding_114": 0.012526587, "title+abstract_embedding_115": -0.06154097, "title+abstract_embedding_116": 0.1423837, "title+abstract_embedding_117": 0.18794823, "title+abstract_embedding_118": 0.007614413, "title+abstract_embedding_119": 0.038617644, "title+abstract_embedding_120": 0.12721856, "title+abstract_embedding_121": -0.09506803, "title+abstract_embedding_122": 0.00502184, "title+abstract_embedding_123": 0.038379945, "title+abstract_embedding_124": 0.11243207, "title+abstract_embedding_125": 0.14980775, "title+abstract_embedding_126": 0.02904046, "title+abstract_embedding_127": -0.092530996, "label": 14, "label-multi": "1;14" }, { "paper_new_id": 39, "id": "j_2f0b74d46eeb895973c9cd8be4a90071", "title+abstract": "Characterization of the hydroperoxyl/superoxide anion radical (HO2/O2a??) formed from the photolysis of immobilized TiO2 in a continuous flow;Abstract In this study, the steady-state concentrations of HO 2 /O 2 ? formed from the photocatalysis of immobilized TiO 2 were investigated quantitatively by using the kinetic method with a continuous flow injection. In air-equilibrated water, the concentration of HO 2 /O 2 ? was typically 1.01 (?¨¤0.08)??¨¢?10 ?9 ?M at pH 5.80 in the absence of buffers. The reduction of O 2 by photo-induced electrons (e cb ? ) was increased by the concentration of O 2 (from 0 to 0.38?mM). However, in the presence of buffer anions the concentration of HO 2 /O 2 ? was gradually decreased by increasing pH. This indicates that the suppression of HO 2 /O 2 ? in the presence of buffer ions is attributed to the blocking of active sites of the immobilized TiO 2 photocatalyst and to certain processes, that is, the reaction between HO 2 /O 2 ? and OH (and/or h vb + ). Furthermore, the concentration of HO 2 /O 2 ? increased with the increasing concentrations of H 2 O 2 and oxalate, and then on the further addition of H 2 O 2 (>10?mM) and oxalate (>2?mM), the concentration of HO 2 /O 2 ? reached steady values. These results strongly suggest that HO 2 /O 2 ? formed on TiO 2 photocatalysis migrates into the water bulk, and this study can contribute significantly to the body of knowledge regarding HO 2 /O 2 ? at very low levels.", "title+abstract_embedding_0": 0.97553074, "title+abstract_embedding_1": 0.093170404, "title+abstract_embedding_2": 1.1533127, "title+abstract_embedding_3": 0.19463146, "title+abstract_embedding_4": 0.6380046, "title+abstract_embedding_5": 0.0989902, "title+abstract_embedding_6": 0.528813, "title+abstract_embedding_7": 0.02434009, "title+abstract_embedding_8": -0.52837306, "title+abstract_embedding_9": 0.111065984, "title+abstract_embedding_10": -0.18332018, "title+abstract_embedding_11": -0.55173206, "title+abstract_embedding_12": -0.2922497, "title+abstract_embedding_13": 0.2648593, "title+abstract_embedding_14": -0.5980299, "title+abstract_embedding_15": -0.063104324, "title+abstract_embedding_16": 0.31108427, "title+abstract_embedding_17": -0.19500569, "title+abstract_embedding_18": -0.47906083, "title+abstract_embedding_19": 0.36681277, "title+abstract_embedding_20": -0.48821193, "title+abstract_embedding_21": -0.10158205, "title+abstract_embedding_22": -0.10854518, "title+abstract_embedding_23": 0.14918387, "title+abstract_embedding_24": 0.46588272, "title+abstract_embedding_25": -0.13091743, "title+abstract_embedding_26": 0.09051865, "title+abstract_embedding_27": -0.262062, "title+abstract_embedding_28": -0.17545134, "title+abstract_embedding_29": 0.17532085, "title+abstract_embedding_30": 0.14971644, "title+abstract_embedding_31": 0.25522283, "title+abstract_embedding_32": 0.19127108, "title+abstract_embedding_33": 0.2847512, "title+abstract_embedding_34": 0.24618046, "title+abstract_embedding_35": -0.07257576, "title+abstract_embedding_36": -0.20425104, "title+abstract_embedding_37": 0.22233285, "title+abstract_embedding_38": 0.3545005, "title+abstract_embedding_39": -0.09981691, "title+abstract_embedding_40": 0.28235412, 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-0.11902908, "title+abstract_embedding_64": -0.029736668, "title+abstract_embedding_65": -0.003226072, "title+abstract_embedding_66": -0.29243472, "title+abstract_embedding_67": -0.14392401, "title+abstract_embedding_68": -0.25195718, "title+abstract_embedding_69": 0.039787106, "title+abstract_embedding_70": -3.7e-05, "title+abstract_embedding_71": -0.12193808, "title+abstract_embedding_72": -0.09472016, "title+abstract_embedding_73": 0.16746925, "title+abstract_embedding_74": -0.23971178, "title+abstract_embedding_75": 0.10680555, "title+abstract_embedding_76": -0.19666961, "title+abstract_embedding_77": 0.20540564, "title+abstract_embedding_78": -0.056035966, "title+abstract_embedding_79": 0.094936945, "title+abstract_embedding_80": 0.004910391, "title+abstract_embedding_81": -0.1526961, "title+abstract_embedding_82": -0.052813083, "title+abstract_embedding_83": 0.03084619, "title+abstract_embedding_84": 0.14258589, "title+abstract_embedding_85": -0.0909667, 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"title+abstract_embedding_108": 0.13716364, "title+abstract_embedding_109": -0.020288944, "title+abstract_embedding_110": -0.11024162, "title+abstract_embedding_111": 0.060266018, "title+abstract_embedding_112": -0.15077825, "title+abstract_embedding_113": -0.16369195, "title+abstract_embedding_114": -0.011047512, "title+abstract_embedding_115": 0.021424621, "title+abstract_embedding_116": -0.070344314, "title+abstract_embedding_117": 0.021717887, "title+abstract_embedding_118": 0.13402782, "title+abstract_embedding_119": 0.05360437, "title+abstract_embedding_120": 0.042559903, "title+abstract_embedding_121": 0.026883554, "title+abstract_embedding_122": 0.08512314, "title+abstract_embedding_123": -0.06820532, "title+abstract_embedding_124": 0.03372384, "title+abstract_embedding_125": -0.14806473, "title+abstract_embedding_126": 0.053345867, "title+abstract_embedding_127": 0.15119004, "label": 3, "label-multi": "3" }, { "paper_new_id": 40, "id": "j_2f6098e02f909180243f88be2cd73758", "title+abstract": "Visible-Light Degradation of Organic Dye Based on a Heterostructure Photocatalyst;Novel highly visible-light active 1.0rGO¡§CZnBi 2 O 4 ¡§CBi 2 S 3 heterostructure photocatalysts with various weight percentages of Bi 2 S 3 were successfully synthesized. First, the 1.0rGO¡§CZnBi 2 O 4 catalyst was synthesized by a simple two-step oxidation¡§Creduction and co-precipitation methods, followed by heating at 450???C. Then, 1.0rGO¡§CZnBi 2 O 4 was hydrothermally treated with Bi 3+ , and thiourea in ethylene glycol to obtain the 1.0rGO¡§CZnBi 2 O 4 ¡§CBi 2 S 3 heterostructure photocatalyst. The obtained 1.0rGO¡§CZnBi 2 O 4 ¡§CBi 2 S 3 heterostructure photocatalysts were characterized by X-ray diffraction, UV¡§CVis diffuse reflectance spectroscopy, scanning electron microscopy, X-ray photoelectron spectroscopy, and Raman spectroscopy. Photocatalytic studies were conducted using Indigo carmine and it was found that the heterostructure photocatalyst enabled an almost complete degradation of the pollutants. The enhanced catalytic activity of the 1.0rGO¡§CZnBi 2 O 4 ¡§C2.0Bi 2 S 3 heterostructure photocatalyst is due to the homogeneous distribution of ZnBi 2 O 4 ¡§C2.0Bi 2 S 3 over rGO as well as to the efficient electron-transfer from Bi 2 S 3 to ZnBi 2 O 4 and finally to rGO. More than 97% of Indigo carmine of 50?mg/L was degraded by 1.0rGO¡§CZnBi 2 O 4 ¡§C2.0Bi 2 S 3 in 75?min of visible light irradiation. The reusability of the 1.0rGO¡§CZnBi 2 O 4 ¡§C2.0Bi 2 S 3 was studied, and after four cycles, the Indigo carmine degradation efficiency decreased to 90%.The mechanism of the Indigo carmine degradation by the 1.0rGO¡§CZnBi 2 O 4 ¡§C2.0Bi 2 S 3 catalysis likely consists of to two main processes: first, charge transfer prolongs the lifetime of the electron¡§Chole pairs, and then the electron¡§Chole pairs participate in the reactions that produce free radicals.", "title+abstract_embedding_0": 0.8751663, "title+abstract_embedding_1": 0.73104095, "title+abstract_embedding_2": 0.7484776, "title+abstract_embedding_3": -0.7465327, "title+abstract_embedding_4": 0.5949355, "title+abstract_embedding_5": -0.53171825, "title+abstract_embedding_6": -0.39013317, "title+abstract_embedding_7": 0.9228132, "title+abstract_embedding_8": -0.5447279, "title+abstract_embedding_9": -0.086999595, "title+abstract_embedding_10": -0.031600215, "title+abstract_embedding_11": -0.062605, 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"title+abstract_embedding_103": 0.14753258, "title+abstract_embedding_104": -0.04593721, "title+abstract_embedding_105": 0.10523981, "title+abstract_embedding_106": -0.007095903, "title+abstract_embedding_107": 0.10067532, "title+abstract_embedding_108": -0.13031422, "title+abstract_embedding_109": 0.041203633, "title+abstract_embedding_110": -0.1262323, "title+abstract_embedding_111": 0.156122, "title+abstract_embedding_112": 0.09259028, "title+abstract_embedding_113": 0.089204416, "title+abstract_embedding_114": -0.016505212, "title+abstract_embedding_115": 0.06023747, "title+abstract_embedding_116": 0.20247982, "title+abstract_embedding_117": 0.10905014, "title+abstract_embedding_118": 0.04467222, "title+abstract_embedding_119": -0.15452692, "title+abstract_embedding_120": -0.031367846, "title+abstract_embedding_121": 0.14941402, "title+abstract_embedding_122": -0.09787929, "title+abstract_embedding_123": -0.11949904, "title+abstract_embedding_124": -0.1114699, "title+abstract_embedding_125": 0.21026361, "title+abstract_embedding_126": 0.064784676, "title+abstract_embedding_127": 0.103883766, "label": 3, "label-multi": "3" }, { "paper_new_id": 41, "id": "j_2fd50ccdbb911bc84809763103d6370f", "title+abstract": "Preparation of C60(O)n-ZnO Nanocomposite Under Electric Furnace and Photocatalytic Degradation of Organic Dyes;Zinc sulfide (ZnS) nanoparticles were synthesized from zinc nitrate hexahydrate and thiourea under microwave irradiation. The ZnS-graphene nanocomposites were calcined in an electric furnace at 700 degrees C under an inert argon gas atmosphere for 2 hr. The heated ZnS-graphene nanocomposites were characterized by X-ray diffraction, scanning electron microscopy, transmission electron microscopy and UV-vis spectrophotometry. After heat treatment, ZnS-graphene nanocomposites had a more porous and larger surface area, than the unheated ZnS-graphene nanocomposites. The photocatalytic activity of the heated ZnS-graphene nanocomposites in the degradation of organic dyes, such as methylene blue, methyl orange, and rhodamine B, under ultraviolet light at 254 nm by UV- vis spectrophotometer was evaluated and compared with that of the unheated ZnS nanoparticles, heated ZnS nanoparticles, unheated ZnS-graphene nanocomposites. Among the our experimental results as a photocatalyst, the heated ZnS-graphene nanocomposites exhibited remarkably higher photocatalytic degradation of organic dyes as compared to other nanomaterials such as unheated ZnS nanoparticles and heated ZnS-graphene nanocomposites.", "title+abstract_embedding_0": 1.145738, "title+abstract_embedding_1": -0.07923165, "title+abstract_embedding_2": -1.8056796, "title+abstract_embedding_3": -0.2284466, "title+abstract_embedding_4": -0.43553907, "title+abstract_embedding_5": -1.3158237, "title+abstract_embedding_6": -0.6113353, "title+abstract_embedding_7": -0.12453452, "title+abstract_embedding_8": 0.62983876, "title+abstract_embedding_9": 0.15543741, "title+abstract_embedding_10": -0.30992454, "title+abstract_embedding_11": -0.60895973, "title+abstract_embedding_12": 0.499235, "title+abstract_embedding_13": -0.10183033, "title+abstract_embedding_14": 0.44057557, "title+abstract_embedding_15": -0.1696469, "title+abstract_embedding_16": 0.14285469, "title+abstract_embedding_17": -0.028647736, "title+abstract_embedding_18": 0.076927826, "title+abstract_embedding_19": 0.58373994, "title+abstract_embedding_20": -0.23879296, "title+abstract_embedding_21": -0.19709197, "title+abstract_embedding_22": 0.44148323, "title+abstract_embedding_23": -0.017890245, "title+abstract_embedding_24": -0.042159095, "title+abstract_embedding_25": 0.1081959, "title+abstract_embedding_26": -0.48843035, "title+abstract_embedding_27": -0.084053844, "title+abstract_embedding_28": -0.18633008, "title+abstract_embedding_29": 0.55223644, "title+abstract_embedding_30": -0.030574888, "title+abstract_embedding_31": -0.03164186, "title+abstract_embedding_32": -0.1648544, "title+abstract_embedding_33": 0.00568983, "title+abstract_embedding_34": 0.057018742, "title+abstract_embedding_35": 0.002807699, "title+abstract_embedding_36": 0.19006181, "title+abstract_embedding_37": 0.04167895, "title+abstract_embedding_38": -0.3066997, "title+abstract_embedding_39": -0.055204935, "title+abstract_embedding_40": 0.27371716, "title+abstract_embedding_41": 0.2789389, "title+abstract_embedding_42": 0.11142561, "title+abstract_embedding_43": 0.034935787, "title+abstract_embedding_44": -0.22769451, "title+abstract_embedding_45": -0.1890529, "title+abstract_embedding_46": 0.17668292, "title+abstract_embedding_47": -0.051578365, "title+abstract_embedding_48": 0.17500576, "title+abstract_embedding_49": -0.07502842, "title+abstract_embedding_50": 0.21869461, "title+abstract_embedding_51": -0.35290003, "title+abstract_embedding_52": -0.065563545, "title+abstract_embedding_53": -0.22130576, "title+abstract_embedding_54": 0.13907595, "title+abstract_embedding_55": -0.21702908, "title+abstract_embedding_56": -0.105103925, "title+abstract_embedding_57": 0.033898056, "title+abstract_embedding_58": -0.24567887, "title+abstract_embedding_59": 0.065588936, "title+abstract_embedding_60": 0.30186814, "title+abstract_embedding_61": 0.043502264, "title+abstract_embedding_62": -0.026090398, "title+abstract_embedding_63": -0.003675353, "title+abstract_embedding_64": 0.14041664, "title+abstract_embedding_65": 0.06435934, "title+abstract_embedding_66": -0.10713214, "title+abstract_embedding_67": 0.13556933, "title+abstract_embedding_68": 0.012866952, "title+abstract_embedding_69": -0.17004041, "title+abstract_embedding_70": 0.08203441, "title+abstract_embedding_71": -0.34021318, "title+abstract_embedding_72": 0.02797602, "title+abstract_embedding_73": 0.11523108, "title+abstract_embedding_74": 0.21179624, "title+abstract_embedding_75": -0.15130508, "title+abstract_embedding_76": -0.21029332, "title+abstract_embedding_77": 0.030392632, "title+abstract_embedding_78": -0.001215838, "title+abstract_embedding_79": -0.18661511, "title+abstract_embedding_80": -0.11814573, "title+abstract_embedding_81": 0.27081475, "title+abstract_embedding_82": -0.15893328, "title+abstract_embedding_83": 2.7260743e-05, "title+abstract_embedding_84": 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"title+abstract_embedding_107": 0.030784214, "title+abstract_embedding_108": 0.08120543, "title+abstract_embedding_109": 0.11627887, "title+abstract_embedding_110": -0.07380919, "title+abstract_embedding_111": -0.032572016, "title+abstract_embedding_112": 0.037078142, "title+abstract_embedding_113": 0.19615681, "title+abstract_embedding_114": 0.02743958, "title+abstract_embedding_115": -0.19364414, "title+abstract_embedding_116": -0.07869163, "title+abstract_embedding_117": 0.06186985, "title+abstract_embedding_118": -0.12889592, "title+abstract_embedding_119": -0.011931084, "title+abstract_embedding_120": -0.0864753, "title+abstract_embedding_121": 0.08578082, "title+abstract_embedding_122": 0.012196928, "title+abstract_embedding_123": -0.1184966, "title+abstract_embedding_124": 0.058161475, "title+abstract_embedding_125": 0.10449429, "title+abstract_embedding_126": 0.01075244, "title+abstract_embedding_127": 0.04849346, "label": 106, "label-multi": NaN }, { "paper_new_id": 42, "id": "j_2fd89a525d65d2877b9674db27e646e0", "title+abstract": "Photocatalytically Active Conjugated Porous Polymers via Click Chemistry for Heterogeneous Dehydrogenation of Hydrazo Aromatics;Aromatic azo compounds are an important class of raw materials and are widely used in chemical industries. However, current synthetic methods have many disadvantages, which limit their practical utility. Here, we report a facile approach to prepare 1,2,3-triazole-contained conjugated porous polymers (CPPs; Ta-Ths) through click reaction of azide and terminal alkynes and employ the click-based CPPs for the first time as photocatalysts. By changing the structure of alkyne monomer, Ta-Ths with distinct optoelectronic properties are obtained to effectively catalyze the visible light-driven oxidative dehydrogenation of hydrazo aromatics. Moreover, the Ta-Ths show much higher catalytic activity as compared with previous homogeneous photocatalysts. The CPP that possesses better charge transfer efficiency and lower charge recombination rate was found to have more catalytic activity than the others. In addition, this protocol was demonstrated on a gram scale without any erosion of yield. Furthermore, the polymer photocatalyst has shown reliable recyclability with no significant loss in its catalytic activity.", "title+abstract_embedding_0": -0.17912292, "title+abstract_embedding_1": 0.7185855, "title+abstract_embedding_2": 0.47783908, "title+abstract_embedding_3": -0.4320153, "title+abstract_embedding_4": -0.43045768, "title+abstract_embedding_5": 0.16862807, "title+abstract_embedding_6": -0.3659697, "title+abstract_embedding_7": 0.233909, "title+abstract_embedding_8": 0.14035685, "title+abstract_embedding_9": 0.38750482, "title+abstract_embedding_10": 0.36976936, "title+abstract_embedding_11": -0.18210468, "title+abstract_embedding_12": 0.38470823, "title+abstract_embedding_13": 0.08914046, "title+abstract_embedding_14": 0.16864282, "title+abstract_embedding_15": 0.30580422, "title+abstract_embedding_16": -0.17808664, "title+abstract_embedding_17": -0.7671932, "title+abstract_embedding_18": 0.026013032, "title+abstract_embedding_19": -0.6081962, "title+abstract_embedding_20": -0.041735463, "title+abstract_embedding_21": 0.4298866, "title+abstract_embedding_22": 0.1030741, "title+abstract_embedding_23": 0.25138867, "title+abstract_embedding_24": -0.011976898, "title+abstract_embedding_25": 0.4065354, "title+abstract_embedding_26": 0.36908898, "title+abstract_embedding_27": 0.007793896, "title+abstract_embedding_28": 0.32141012, "title+abstract_embedding_29": -0.015704429, "title+abstract_embedding_30": -0.37708777, "title+abstract_embedding_31": 0.07450457, "title+abstract_embedding_32": 0.20837739, "title+abstract_embedding_33": 0.2430217, "title+abstract_embedding_34": 0.07482153, "title+abstract_embedding_35": 0.21686724, "title+abstract_embedding_36": 0.07603496, "title+abstract_embedding_37": 0.09958877, "title+abstract_embedding_38": 0.24465668, "title+abstract_embedding_39": 0.007017283, "title+abstract_embedding_40": -0.13048705, "title+abstract_embedding_41": 0.21451013, "title+abstract_embedding_42": 0.14307263, "title+abstract_embedding_43": 0.00332889, "title+abstract_embedding_44": -0.07594441, "title+abstract_embedding_45": 0.1562987, "title+abstract_embedding_46": -0.11425412, "title+abstract_embedding_47": 0.005028777, "title+abstract_embedding_48": 0.078153, "title+abstract_embedding_49": 0.11678085, "title+abstract_embedding_50": 0.1927069, "title+abstract_embedding_51": -0.014067888, "title+abstract_embedding_52": -0.012496479, "title+abstract_embedding_53": -0.17810827, "title+abstract_embedding_54": -0.0794828, "title+abstract_embedding_55": -0.092212945, "title+abstract_embedding_56": -0.036632244, "title+abstract_embedding_57": 0.17718807, "title+abstract_embedding_58": 0.3007428, "title+abstract_embedding_59": 0.05295019, "title+abstract_embedding_60": -0.038817704, "title+abstract_embedding_61": 0.035617523, "title+abstract_embedding_62": -0.02992092, "title+abstract_embedding_63": -0.25875768, "title+abstract_embedding_64": 0.07335316, "title+abstract_embedding_65": -0.23952672, "title+abstract_embedding_66": 0.08889152, "title+abstract_embedding_67": 0.15309745, "title+abstract_embedding_68": -0.07407353, "title+abstract_embedding_69": -0.17812613, "title+abstract_embedding_70": -0.15081123, "title+abstract_embedding_71": 0.05126144, "title+abstract_embedding_72": -0.2703468, "title+abstract_embedding_73": -0.053247046, "title+abstract_embedding_74": 0.009499557, "title+abstract_embedding_75": -0.006426346, "title+abstract_embedding_76": 0.0656251, "title+abstract_embedding_77": -0.14985077, "title+abstract_embedding_78": -0.026399203, "title+abstract_embedding_79": -0.22911409, "title+abstract_embedding_80": 0.012596149, "title+abstract_embedding_81": -0.12443709, "title+abstract_embedding_82": 0.007261634, "title+abstract_embedding_83": 0.15034427, "title+abstract_embedding_84": 0.06720926, "title+abstract_embedding_85": -0.27209944, "title+abstract_embedding_86": 0.053749807, "title+abstract_embedding_87": 0.14283088, "title+abstract_embedding_88": -0.17168367, "title+abstract_embedding_89": -0.13741946, "title+abstract_embedding_90": -0.041261695, "title+abstract_embedding_91": -0.21600708, "title+abstract_embedding_92": 0.0542828, "title+abstract_embedding_93": 0.1698106, "title+abstract_embedding_94": 0.12974691, "title+abstract_embedding_95": -0.08559691, "title+abstract_embedding_96": 0.026521228, "title+abstract_embedding_97": 0.045980193, "title+abstract_embedding_98": 0.07713008, "title+abstract_embedding_99": 0.0788093, "title+abstract_embedding_100": 0.04558704, "title+abstract_embedding_101": -0.22377628, "title+abstract_embedding_102": -0.15643668, "title+abstract_embedding_103": -0.08199822, "title+abstract_embedding_104": 0.17922899, "title+abstract_embedding_105": 0.036435805, "title+abstract_embedding_106": -0.021068528, "title+abstract_embedding_107": -0.108979024, "title+abstract_embedding_108": -0.06554568, "title+abstract_embedding_109": -0.02947706, "title+abstract_embedding_110": -0.08563152, "title+abstract_embedding_111": 0.050806, "title+abstract_embedding_112": -0.008250117, "title+abstract_embedding_113": -0.019383654, "title+abstract_embedding_114": 0.046300724, "title+abstract_embedding_115": 0.003404744, "title+abstract_embedding_116": 0.017096192, "title+abstract_embedding_117": -0.003912911, "title+abstract_embedding_118": -0.059894495, "title+abstract_embedding_119": 0.026457775, "title+abstract_embedding_120": -0.000607515, "title+abstract_embedding_121": -0.09571449, "title+abstract_embedding_122": 0.036793172, "title+abstract_embedding_123": 0.20087522, "title+abstract_embedding_124": -0.03800442, "title+abstract_embedding_125": 0.073528014, "title+abstract_embedding_126": -0.14477693, "title+abstract_embedding_127": 0.1865276, "label": 3, "label-multi": "0;19;3" }, { "paper_new_id": 43, "id": "j_3224470ba90441f2038065419af13de5", "title+abstract": "Photocatalytic degradation of an organic pollutant by zinc oxide a?? solar process;Abstract The photocatalytic degradation of 4-nitrophenol over irradiated ZnO suspensions was investigated in aerated aqueous solution. Complete degradation was achieved after irradiation with solar light, being the reaction rate dependent on the initial pH. The effect of various parameters such as catalyst loading, pH and initial concentration of 4-nitrophenol on degradation has been determined. The degradation was strongly enhanced in the presence of electron acceptors such as H2O2, K2S2O8 and KBrO3. The kinetics of heterogeneous photocatalytic degradation is discussed interms of Langmuir¡§CHinshelwood (L¡§CH) kinetic model. The intermediates formed during the photodegradation were identified by GC¡§CMS analysis. The mineralization of 4-nitrophenol has also been confirmed by COD measurements.", "title+abstract_embedding_0": -0.12145746, "title+abstract_embedding_1": 1.4678496, "title+abstract_embedding_2": 1.1395217, "title+abstract_embedding_3": 0.07647973, "title+abstract_embedding_4": -0.20303601, "title+abstract_embedding_5": -1.253013, "title+abstract_embedding_6": -0.24480304, "title+abstract_embedding_7": 0.08126646, "title+abstract_embedding_8": 0.4212463, "title+abstract_embedding_9": 0.016196609, "title+abstract_embedding_10": -0.36724335, "title+abstract_embedding_11": -0.15134507, "title+abstract_embedding_12": 0.128851, "title+abstract_embedding_13": -0.11133889, "title+abstract_embedding_14": 0.55824184, "title+abstract_embedding_15": -0.1707843, "title+abstract_embedding_16": 0.41797388, "title+abstract_embedding_17": -0.34847683, "title+abstract_embedding_18": -0.2176261, "title+abstract_embedding_19": 0.19192049, "title+abstract_embedding_20": 0.35305864, "title+abstract_embedding_21": -0.07279241, "title+abstract_embedding_22": 0.14056781, "title+abstract_embedding_23": 0.0961898, "title+abstract_embedding_24": -0.2567013, "title+abstract_embedding_25": 0.4778365, "title+abstract_embedding_26": -0.07349992, "title+abstract_embedding_27": 0.33138868, "title+abstract_embedding_28": -0.13181612, "title+abstract_embedding_29": -0.034563504, "title+abstract_embedding_30": 0.14500591, "title+abstract_embedding_31": -0.55089617, "title+abstract_embedding_32": -0.0740559, "title+abstract_embedding_33": -0.20838952, "title+abstract_embedding_34": 0.10240949, "title+abstract_embedding_35": -0.046074487, "title+abstract_embedding_36": -0.1043108, "title+abstract_embedding_37": 0.2836783, "title+abstract_embedding_38": -0.047595438, "title+abstract_embedding_39": -0.28911948, "title+abstract_embedding_40": -0.23394585, "title+abstract_embedding_41": -0.060608897, "title+abstract_embedding_42": 0.012482077, "title+abstract_embedding_43": -0.041002154, "title+abstract_embedding_44": -0.14501211, "title+abstract_embedding_45": 0.10876307, "title+abstract_embedding_46": 0.14162782, "title+abstract_embedding_47": 0.051458392, "title+abstract_embedding_48": 0.22641167, "title+abstract_embedding_49": -0.018686526, "title+abstract_embedding_50": -0.07348687, "title+abstract_embedding_51": 0.10887662, "title+abstract_embedding_52": -0.011792466, "title+abstract_embedding_53": -0.194563, "title+abstract_embedding_54": -0.20770963, "title+abstract_embedding_55": -0.28781706, "title+abstract_embedding_56": 0.37348574, "title+abstract_embedding_57": -0.14236033, "title+abstract_embedding_58": -0.1301373, "title+abstract_embedding_59": -0.05021645, "title+abstract_embedding_60": 0.00723359, "title+abstract_embedding_61": -0.09943589, "title+abstract_embedding_62": -0.02489565, "title+abstract_embedding_63": -0.005213257, "title+abstract_embedding_64": -0.22095235, "title+abstract_embedding_65": -0.12355368, "title+abstract_embedding_66": -0.029563636, "title+abstract_embedding_67": -0.17615378, "title+abstract_embedding_68": 0.14451665, "title+abstract_embedding_69": 0.15001833, "title+abstract_embedding_70": 0.048518065, "title+abstract_embedding_71": -0.013283208, "title+abstract_embedding_72": 0.116863765, "title+abstract_embedding_73": 0.09849497, "title+abstract_embedding_74": 0.06187573, "title+abstract_embedding_75": 0.064998515, "title+abstract_embedding_76": -0.15646034, "title+abstract_embedding_77": -0.048337415, "title+abstract_embedding_78": -0.13721393, "title+abstract_embedding_79": 0.17953789, "title+abstract_embedding_80": 0.09757854, "title+abstract_embedding_81": -0.03775256, "title+abstract_embedding_82": -0.05745378, "title+abstract_embedding_83": 0.01711358, "title+abstract_embedding_84": -0.15604274, "title+abstract_embedding_85": 0.08793413, "title+abstract_embedding_86": -0.007715106, "title+abstract_embedding_87": -0.12093088, "title+abstract_embedding_88": 0.27037334, "title+abstract_embedding_89": 0.018207155, "title+abstract_embedding_90": 0.0756189, "title+abstract_embedding_91": -0.008650623, "title+abstract_embedding_92": -0.14424586, "title+abstract_embedding_93": 0.14679769, "title+abstract_embedding_94": 0.07293187, "title+abstract_embedding_95": 0.003238656, "title+abstract_embedding_96": -0.027236603, "title+abstract_embedding_97": -0.24083069, "title+abstract_embedding_98": 0.13019195, "title+abstract_embedding_99": -0.105571955, "title+abstract_embedding_100": -0.15122208, "title+abstract_embedding_101": 0.0686235, "title+abstract_embedding_102": -0.070007294, "title+abstract_embedding_103": -0.15095466, "title+abstract_embedding_104": -0.043857113, "title+abstract_embedding_105": 0.10288727, "title+abstract_embedding_106": 0.22392753, "title+abstract_embedding_107": 0.110824905, "title+abstract_embedding_108": 0.16908942, "title+abstract_embedding_109": 0.19882335, "title+abstract_embedding_110": -0.13098449, "title+abstract_embedding_111": -0.119124144, "title+abstract_embedding_112": 0.00136739, "title+abstract_embedding_113": 0.07670296, "title+abstract_embedding_114": -0.16940722, "title+abstract_embedding_115": -0.020883262, "title+abstract_embedding_116": -0.11483738, "title+abstract_embedding_117": 0.026487458, "title+abstract_embedding_118": 0.03325656, "title+abstract_embedding_119": -0.046482794, "title+abstract_embedding_120": 0.009898428, "title+abstract_embedding_121": -0.11938806, "title+abstract_embedding_122": 0.0301103, "title+abstract_embedding_123": -0.025547665, "title+abstract_embedding_124": 0.08999861, "title+abstract_embedding_125": 0.0665685, "title+abstract_embedding_126": 0.030260626, "title+abstract_embedding_127": 0.042919092, "label": 3, "label-multi": "3" }, { "paper_new_id": 44, "id": "j_32cfec6bfeb578293fa4ba87bc9868e2", "title+abstract": "Single layer of nickel hydroxide nanoparticles covered on a porous Ni foam and its application for highly sensitive non-enzymatic glucose sensor;Abstract A single layer of nickel hydroxide nanoparticles (Ni(OH)2 NPs) was covered on the full surface of a porous Ni foam by simply applying an electrochemical cyclic voltammetric (CV) treatment on a bare Ni foam substrate for 100 cycles in 1.0?M NaOH solution. The surface morphology of the obtained Ni(OH)2 NPs/Ni foam electrode was examined by scanning electron microscopy. The thickness of the Ni(OH)2 NPs layer on the electrode was estimated by X-ray photoelectron spectroscopy with Ar+ ion etching. In CV measurement, the Ni(OH)2 NPs/Ni foam electrode exhibited excellent electrocatalytic ability toward glucose in NaOH solution. The Ni(OH)2 NPs/Ni foam electrode was successfully used for the quantification of glucose by an amperometric method. The sensing parameters include a high sensitivity of 1950.3?|¨¬A/mM-cm2, a linear range from 0.6 to 6.0?mM, a detection limit of 0.16?|¨¬M, and an applied potential of 0.45?V (vs. Ag/AgCl/KCl sat?¡¥d). The excellent performances obtained in the interference test, the long-term durability test in atmosphere, and the reproducibility test of the Ni(OH)2 NPs/Ni foam sensor indicate the applicability of the proposed electrode as a reliable non-enzymatic glucose sensor.", "title+abstract_embedding_0": 0.22264993, "title+abstract_embedding_1": -1.6088265, "title+abstract_embedding_2": -0.4373853, "title+abstract_embedding_3": 0.51729107, "title+abstract_embedding_4": -0.09608841, "title+abstract_embedding_5": -0.8338162, "title+abstract_embedding_6": 0.44835144, "title+abstract_embedding_7": -0.11757672, "title+abstract_embedding_8": -0.74165666, "title+abstract_embedding_9": -0.2418744, "title+abstract_embedding_10": 0.22860628, "title+abstract_embedding_11": -0.021521248, "title+abstract_embedding_12": -0.48346004, "title+abstract_embedding_13": 0.508913, "title+abstract_embedding_14": 0.15029481, "title+abstract_embedding_15": 0.65989536, "title+abstract_embedding_16": 0.007688701, "title+abstract_embedding_17": -0.004277319, "title+abstract_embedding_18": -0.3860389, "title+abstract_embedding_19": 0.004962919, "title+abstract_embedding_20": -0.25021675, "title+abstract_embedding_21": 0.32783058, "title+abstract_embedding_22": -0.022885656, "title+abstract_embedding_23": -0.30644035, "title+abstract_embedding_24": -0.19083661, "title+abstract_embedding_25": 0.15244281, "title+abstract_embedding_26": -0.2804, "title+abstract_embedding_27": -0.43324494, "title+abstract_embedding_28": -0.031918675, "title+abstract_embedding_29": -0.23005544, "title+abstract_embedding_30": -0.02616033, "title+abstract_embedding_31": 0.083927296, "title+abstract_embedding_32": -0.06974503, "title+abstract_embedding_33": 0.041474074, "title+abstract_embedding_34": 0.033633694, "title+abstract_embedding_35": -0.2409482, "title+abstract_embedding_36": -0.07053399, "title+abstract_embedding_37": 0.13725083, "title+abstract_embedding_38": 0.29517263, "title+abstract_embedding_39": 0.012949017, "title+abstract_embedding_40": 0.17407732, "title+abstract_embedding_41": -0.34919682, "title+abstract_embedding_42": -0.040203795, "title+abstract_embedding_43": -0.10722786, "title+abstract_embedding_44": -0.044682994, "title+abstract_embedding_45": 0.08939555, "title+abstract_embedding_46": -0.095584154, "title+abstract_embedding_47": 0.031729277, "title+abstract_embedding_48": -0.21038976, "title+abstract_embedding_49": -0.09172277, "title+abstract_embedding_50": -0.122438066, "title+abstract_embedding_51": -0.2673263, "title+abstract_embedding_52": 0.15857576, "title+abstract_embedding_53": -0.017528877, "title+abstract_embedding_54": -0.30627948, "title+abstract_embedding_55": 0.14039615, "title+abstract_embedding_56": 0.09553069, "title+abstract_embedding_57": 0.14875948, "title+abstract_embedding_58": -0.152799, "title+abstract_embedding_59": 0.025723994, "title+abstract_embedding_60": 0.21615063, "title+abstract_embedding_61": 0.047390822, "title+abstract_embedding_62": 0.023944044, "title+abstract_embedding_63": -0.16422835, "title+abstract_embedding_64": -0.12431981, "title+abstract_embedding_65": -0.06326275, "title+abstract_embedding_66": -0.07903733, "title+abstract_embedding_67": 0.004328519, "title+abstract_embedding_68": -0.046936333, "title+abstract_embedding_69": -0.21718156, "title+abstract_embedding_70": 0.09654993, "title+abstract_embedding_71": 0.114222124, "title+abstract_embedding_72": 0.13146064, "title+abstract_embedding_73": 0.0728062, "title+abstract_embedding_74": -0.2666456, "title+abstract_embedding_75": -0.18372875, "title+abstract_embedding_76": -0.100259274, "title+abstract_embedding_77": -0.10686298, "title+abstract_embedding_78": -0.22691217, "title+abstract_embedding_79": 0.15173711, "title+abstract_embedding_80": -0.28169727, "title+abstract_embedding_81": -0.12788656, "title+abstract_embedding_82": -0.13998568, "title+abstract_embedding_83": -0.19503303, "title+abstract_embedding_84": -0.09091444, "title+abstract_embedding_85": -0.011731843, "title+abstract_embedding_86": 0.20857486, "title+abstract_embedding_87": 0.026257265, "title+abstract_embedding_88": -0.1209701, "title+abstract_embedding_89": -0.017726198, "title+abstract_embedding_90": -0.083191894, "title+abstract_embedding_91": -0.01486554, "title+abstract_embedding_92": -0.122189045, "title+abstract_embedding_93": -0.12950888, "title+abstract_embedding_94": -0.004682742, "title+abstract_embedding_95": 0.15244235, "title+abstract_embedding_96": 0.003851481, "title+abstract_embedding_97": -0.028005317, "title+abstract_embedding_98": -0.08425318, "title+abstract_embedding_99": 0.004890762, "title+abstract_embedding_100": 0.07438734, "title+abstract_embedding_101": -0.16116534, "title+abstract_embedding_102": 0.028797373, "title+abstract_embedding_103": 0.033064216, "title+abstract_embedding_104": -0.219621, "title+abstract_embedding_105": 0.009638533, "title+abstract_embedding_106": -0.122024536, "title+abstract_embedding_107": 0.042452, "title+abstract_embedding_108": -0.12260088, "title+abstract_embedding_109": -0.02150774, "title+abstract_embedding_110": -0.08129285, "title+abstract_embedding_111": 0.057599023, "title+abstract_embedding_112": 0.16165443, "title+abstract_embedding_113": -0.12768586, "title+abstract_embedding_114": -0.017546535, "title+abstract_embedding_115": 0.13495752, "title+abstract_embedding_116": 0.06561459, "title+abstract_embedding_117": -0.09214312, "title+abstract_embedding_118": -0.001088843, "title+abstract_embedding_119": -0.060168844, "title+abstract_embedding_120": -0.07674286, "title+abstract_embedding_121": -0.08565991, "title+abstract_embedding_122": -0.05009997, "title+abstract_embedding_123": 0.10336772, "title+abstract_embedding_124": -0.09059527, "title+abstract_embedding_125": 0.1183147, "title+abstract_embedding_126": 0.096997574, "title+abstract_embedding_127": -0.14164406, "label": 3, "label-multi": "14;24;3" }, { "paper_new_id": 45, "id": "j_330a937888db827bd976174ffc195100", "title+abstract": "Ag Nanoparticle Embedded TiO2 Composite Nanorod Arrays Fabricated by Oblique Angle Deposition: Toward Plasmonic Photocatalysis;Using a unique oblique angle co-deposition technique, well-aligned arrays of Ag nanoparticle embedded TiO2 composite nanorods have been fabricated with different concentrations of Ag. The structural, optical, and photocatalytic properties of the composite nanostructures are investigated using a variety of experimental techniques and compared with those of pure TiO2 nanorods fabricated similarly. Ag nanoparticles are formed in the composite nanorods, which increase the visible light absorbance due to localized surface plasmon resonance. The Ag concentrations and the annealing conditions are found to affect the size and the density of Ag nanoparticles and their optical properties. The Ag nanoparticle embedded TiO2 nanostructures exhibit enhanced photocatalytic activity compared to pure TiO2 under visible- or UV-light illumination. Ag plays different roles in assisting the photocatalysis with different light sources. Ag can be excited and can inject electrons to TiO2, working as an electron donor under visible light. While under UV illumination, Ag acts as an electron acceptor to trap the photogenerated electrons in TiO2. Due to the opposite electron transfer direction under UV and visible light, the presence of Ag may not result in a greater enhancement in the photocatalytic performance.", "title+abstract_embedding_0": 0.74014866, "title+abstract_embedding_1": 0.40039116, "title+abstract_embedding_2": -1.2721123, "title+abstract_embedding_3": 0.2523116, "title+abstract_embedding_4": 0.273637, "title+abstract_embedding_5": 0.4796818, "title+abstract_embedding_6": 0.21195716, "title+abstract_embedding_7": -0.2414209, "title+abstract_embedding_8": -0.42761597, "title+abstract_embedding_9": -0.13247561, "title+abstract_embedding_10": 0.09992728, "title+abstract_embedding_11": 1.3051655, "title+abstract_embedding_12": 0.18867092, "title+abstract_embedding_13": 0.22490445, "title+abstract_embedding_14": -0.32869816, "title+abstract_embedding_15": 0.3346636, "title+abstract_embedding_16": -0.22620595, "title+abstract_embedding_17": -0.18440442, "title+abstract_embedding_18": -0.050293557, "title+abstract_embedding_19": 0.4450566, "title+abstract_embedding_20": 0.1528778, "title+abstract_embedding_21": 0.1172066, "title+abstract_embedding_22": -0.033118766, "title+abstract_embedding_23": 0.6920978, "title+abstract_embedding_24": 0.5225264, "title+abstract_embedding_25": -0.11981189, "title+abstract_embedding_26": -0.54262435, "title+abstract_embedding_27": 0.056083534, "title+abstract_embedding_28": 0.052077904, "title+abstract_embedding_29": -0.021841409, "title+abstract_embedding_30": -0.062300056, "title+abstract_embedding_31": 0.49240118, "title+abstract_embedding_32": -0.22789669, "title+abstract_embedding_33": 0.028605834, "title+abstract_embedding_34": 0.095994756, "title+abstract_embedding_35": 0.11912461, "title+abstract_embedding_36": 0.41794166, "title+abstract_embedding_37": 0.29590678, "title+abstract_embedding_38": 0.03586764, "title+abstract_embedding_39": -0.4028509, "title+abstract_embedding_40": 0.11302826, "title+abstract_embedding_41": 0.14346366, "title+abstract_embedding_42": 0.12496936, "title+abstract_embedding_43": -0.34383485, "title+abstract_embedding_44": -0.09578112, "title+abstract_embedding_45": 0.22185087, "title+abstract_embedding_46": 0.28116447, "title+abstract_embedding_47": 0.036105264, "title+abstract_embedding_48": -0.025268227, "title+abstract_embedding_49": -0.06310463, "title+abstract_embedding_50": -0.016318545, "title+abstract_embedding_51": -0.17136559, "title+abstract_embedding_52": -0.2628016, "title+abstract_embedding_53": -0.042539448, "title+abstract_embedding_54": -0.25304645, "title+abstract_embedding_55": 0.048249707, "title+abstract_embedding_56": -0.3341811, "title+abstract_embedding_57": -0.020355925, "title+abstract_embedding_58": -0.1474023, "title+abstract_embedding_59": -0.09545864, "title+abstract_embedding_60": -0.105038404, "title+abstract_embedding_61": 0.05112876, "title+abstract_embedding_62": -0.030125055, "title+abstract_embedding_63": -0.2596513, "title+abstract_embedding_64": -0.055322304, "title+abstract_embedding_65": 0.023098752, "title+abstract_embedding_66": 0.061605636, "title+abstract_embedding_67": -0.22064137, "title+abstract_embedding_68": 0.16022544, "title+abstract_embedding_69": 0.0157535, "title+abstract_embedding_70": -0.22482964, "title+abstract_embedding_71": 0.015985966, "title+abstract_embedding_72": 0.09118477, "title+abstract_embedding_73": -0.062001403, "title+abstract_embedding_74": 0.012826785, "title+abstract_embedding_75": -0.27272516, "title+abstract_embedding_76": 0.04947251, "title+abstract_embedding_77": -0.004368335, "title+abstract_embedding_78": 0.17330502, "title+abstract_embedding_79": 0.085260615, "title+abstract_embedding_80": -0.05816602, "title+abstract_embedding_81": 0.034600753, "title+abstract_embedding_82": 0.06279962, "title+abstract_embedding_83": 0.07608059, "title+abstract_embedding_84": 0.24003589, "title+abstract_embedding_85": 0.011226961, "title+abstract_embedding_86": 0.047614746, "title+abstract_embedding_87": 0.07251778, "title+abstract_embedding_88": -0.10891293, "title+abstract_embedding_89": -0.0949237, "title+abstract_embedding_90": 0.021484315, "title+abstract_embedding_91": -0.09717331, "title+abstract_embedding_92": 0.10945512, "title+abstract_embedding_93": -0.13062748, "title+abstract_embedding_94": 0.14965087, "title+abstract_embedding_95": 0.017682776, "title+abstract_embedding_96": 0.051929343, "title+abstract_embedding_97": 0.09542014, "title+abstract_embedding_98": 0.22786859, "title+abstract_embedding_99": -0.002516463, "title+abstract_embedding_100": -0.049027443, "title+abstract_embedding_101": 0.012533426, "title+abstract_embedding_102": 0.015866987, "title+abstract_embedding_103": 0.1043413, "title+abstract_embedding_104": 0.009387314, "title+abstract_embedding_105": -0.043754436, "title+abstract_embedding_106": -0.024474487, "title+abstract_embedding_107": 0.098568894, "title+abstract_embedding_108": -0.040174264, "title+abstract_embedding_109": -0.031018034, "title+abstract_embedding_110": 0.299439, "title+abstract_embedding_111": 0.027802065, "title+abstract_embedding_112": 0.22457112, "title+abstract_embedding_113": 0.06515874, "title+abstract_embedding_114": 0.112160236, "title+abstract_embedding_115": 0.07832043, "title+abstract_embedding_116": -0.09755194, "title+abstract_embedding_117": -0.01763989, "title+abstract_embedding_118": -0.06244137, "title+abstract_embedding_119": -0.2741531, "title+abstract_embedding_120": 0.06465702, "title+abstract_embedding_121": -0.24185473, "title+abstract_embedding_122": -0.057442695, "title+abstract_embedding_123": 0.004002973, "title+abstract_embedding_124": -0.036929063, "title+abstract_embedding_125": 0.08226313, "title+abstract_embedding_126": 0.1107467, "title+abstract_embedding_127": 0.051102765, "label": 1, "label-multi": "1;15" }, { "paper_new_id": 46, "id": "j_363b3d46084dd3c42b2a216b04da7a22", "title+abstract": "Enhanced photo catalytic reduction of Cr (VI) over polymer-sensitized g-C3N4/ZnFe2O4 and its synergism with phenol oxidation under visible light irradiation;Abstract A polymer-sensitized g-C3N4/ZnFe2O4 photocatalyst was prepared by in situ calcinations followed by loading of PANI by physisorptions and in situ oxidative polymerization method. The synthesized nanocomposites were characterized by using XRD, FTIR, UV¡§Cvis DRS, XPS, PL, SEM and TEM analysis. A good coordination between CN, ZF and PANI was confirmed from FTIR as well as TEM images. The visible light active PANI-sensitized g-C3N4/ZnFe2O4 heterostructure was used for the photoreduction of Cr (VI) and the photooxidation of phenol simultaneously. However, the photocatalytic reduction of Cr (VI) occurs more rapidly for the coexistence system of phenol and Cr(VI) in comparison to single species, showing synergetic effect. Furthermore, it was found that PANI exhibits excellent photosensitization effect to enhance light absorption. The enhanced photo catalytic activity of PANI-sensitized g-C3N4/ZnFe2O4 photocatalyst is in good agreement with the obtained photocurrent results. PANI-sensitized g-C3N4/ZnFe2O4 photocatalyst gives an anodic photocurrent density of 2.5?mA/cm2 and cathodic current of ?1.6?mA/cm2, which is much more than that of the neat counterparts. The first-order kinetic constant of photo catalytic Cr(VI) reduction in presence of phenol was 0.0324?min?1, being about three times more than that for the reduction of single species chromium. The results obtained from this study illustrate that the prepared PANI-sensitized g-C3N4/ZnFe2O4 photocatalyst can be very well used as an effective and economically viable catalyst due to the ease of separation, and for simultaneous removal of toxic contaminants like Cr(VI) and phenol from wastewater. This magnetic based semiconductor photocatalyst is of great concern to overcome the problem of separation and secondary pollution. This method can also be highly desirable for environmental remediation due to the use of no additional scavengers in this process.", "title+abstract_embedding_0": 0.7884289, "title+abstract_embedding_1": 0.7926327, "title+abstract_embedding_2": 0.06966451, "title+abstract_embedding_3": -0.74194574, "title+abstract_embedding_4": 0.05014378, "title+abstract_embedding_5": -0.24550653, "title+abstract_embedding_6": -0.79416513, "title+abstract_embedding_7": 0.45798904, "title+abstract_embedding_8": 0.25392696, "title+abstract_embedding_9": -0.28544074, "title+abstract_embedding_10": -0.24049208, "title+abstract_embedding_11": -0.11373418, "title+abstract_embedding_12": 0.33892208, "title+abstract_embedding_13": 0.2649913, "title+abstract_embedding_14": -0.4239566, "title+abstract_embedding_15": 0.2570493, "title+abstract_embedding_16": -0.26498514, "title+abstract_embedding_17": -0.20789966, "title+abstract_embedding_18": -0.16633733, "title+abstract_embedding_19": -0.21557817, 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"title+abstract_embedding_88": 0.10059491, "title+abstract_embedding_89": 0.16218388, "title+abstract_embedding_90": -0.07411734, "title+abstract_embedding_91": 0.000953756, "title+abstract_embedding_92": -0.003187761, "title+abstract_embedding_93": 0.24570209, "title+abstract_embedding_94": 0.098453715, "title+abstract_embedding_95": -0.15243793, "title+abstract_embedding_96": -0.010403782, "title+abstract_embedding_97": 0.01625601, "title+abstract_embedding_98": -0.045984924, "title+abstract_embedding_99": 0.18371382, "title+abstract_embedding_100": -0.02239944, "title+abstract_embedding_101": 0.04854019, "title+abstract_embedding_102": -0.05919546, "title+abstract_embedding_103": 0.023679227, "title+abstract_embedding_104": -0.04450901, "title+abstract_embedding_105": 0.019801356, "title+abstract_embedding_106": -0.11088738, "title+abstract_embedding_107": 0.19868286, "title+abstract_embedding_108": 0.015144624, "title+abstract_embedding_109": 0.04980071, "title+abstract_embedding_110": -0.08509846, "title+abstract_embedding_111": -0.048041236, "title+abstract_embedding_112": -0.14817964, "title+abstract_embedding_113": -0.013403595, "title+abstract_embedding_114": -0.01961629, "title+abstract_embedding_115": -0.018741056, "title+abstract_embedding_116": 0.10865061, "title+abstract_embedding_117": 0.061963692, "title+abstract_embedding_118": 0.15775219, "title+abstract_embedding_119": 0.07819666, "title+abstract_embedding_120": -0.06990258, "title+abstract_embedding_121": 0.000640724, "title+abstract_embedding_122": 0.027114287, "title+abstract_embedding_123": 0.042522065, "title+abstract_embedding_124": -0.08067808, "title+abstract_embedding_125": 0.07695637, "title+abstract_embedding_126": 0.01607396, "title+abstract_embedding_127": -0.15594643, "label": 3, "label-multi": "0;3" }, { "paper_new_id": 47, "id": "j_38e22dbda9e4920bd780d12e819dac98", "title+abstract": "Facile Fabrication and High Photoelectric Properties of Hierarchically Ordered Porous TiO2;This paper presents the first successful fabrication of hierarchically ordered porous (HOP) TiO2. Poly(styrene-co-acrylic acid) colloidal spheres and triblock copolymer P123 were used as macro- and mesoporous structure-directing agents, and titanium chloride and titanium tetraisopropoxide were used as sources of titania. When the mixture of polymer spheres, P123, and titania precursors were cast on substrates, and conducted for complete solvent evaporation, followed by thermal treatment, large-scale HOP TiO2 can be directly fabricated. The in situ chelate effect between the titania precursors and the poly(styrene-co-acrylic acid) plays a key role in the fabrication of HOP TiO2. The as-obtained HOP TiO2 exhibits 50% and 70% greater the highest photocurrent under UV and visible lights, respectively, and far higher photoelectrocatalytic property than commercial TiO2 (P-25).", "title+abstract_embedding_0": 0.14244747, "title+abstract_embedding_1": 0.39903504, "title+abstract_embedding_2": -0.39968804, "title+abstract_embedding_3": 1.2199751, "title+abstract_embedding_4": 0.6647015, "title+abstract_embedding_5": 0.71651393, "title+abstract_embedding_6": 0.18451348, "title+abstract_embedding_7": 0.07789558, "title+abstract_embedding_8": 0.2159181, "title+abstract_embedding_9": 0.44104412, "title+abstract_embedding_10": 0.371062, "title+abstract_embedding_11": -0.20307429, "title+abstract_embedding_12": -0.30948737, "title+abstract_embedding_13": 0.29630432, "title+abstract_embedding_14": -0.11915423, "title+abstract_embedding_15": 0.09919932, "title+abstract_embedding_16": -0.23446804, "title+abstract_embedding_17": -0.1944283, "title+abstract_embedding_18": 0.3836068, "title+abstract_embedding_19": -0.12280598, "title+abstract_embedding_20": 0.31663734, "title+abstract_embedding_21": -0.21206523, "title+abstract_embedding_22": -0.14289902, "title+abstract_embedding_23": 0.042143613, "title+abstract_embedding_24": 0.3246147, "title+abstract_embedding_25": -0.21895558, "title+abstract_embedding_26": 0.014949217, "title+abstract_embedding_27": -0.10903831, "title+abstract_embedding_28": 0.19974004, "title+abstract_embedding_29": -0.16545604, "title+abstract_embedding_30": -0.23278114, "title+abstract_embedding_31": 0.034652505, "title+abstract_embedding_32": 0.048595965, "title+abstract_embedding_33": -0.32833844, "title+abstract_embedding_34": 0.03936915, "title+abstract_embedding_35": -0.21364129, "title+abstract_embedding_36": 0.26078779, "title+abstract_embedding_37": -0.3045607, "title+abstract_embedding_38": 0.20854607, "title+abstract_embedding_39": 0.45473033, "title+abstract_embedding_40": -0.35703337, "title+abstract_embedding_41": 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"title+abstract_embedding_64": 0.101324394, "title+abstract_embedding_65": 0.044260472, "title+abstract_embedding_66": 0.26584828, "title+abstract_embedding_67": -0.30188298, "title+abstract_embedding_68": 0.01996088, "title+abstract_embedding_69": -0.31497025, "title+abstract_embedding_70": -0.07885856, "title+abstract_embedding_71": 0.030382693, "title+abstract_embedding_72": 0.19053179, "title+abstract_embedding_73": -0.20487797, "title+abstract_embedding_74": 0.22519489, "title+abstract_embedding_75": 0.07809006, "title+abstract_embedding_76": 0.13191026, "title+abstract_embedding_77": 0.0836307, "title+abstract_embedding_78": -0.09929925, "title+abstract_embedding_79": -0.03243114, "title+abstract_embedding_80": -0.06292529, "title+abstract_embedding_81": 0.080299236, "title+abstract_embedding_82": 0.11582877, "title+abstract_embedding_83": 0.104039215, "title+abstract_embedding_84": -0.21480884, "title+abstract_embedding_85": -0.15829997, "title+abstract_embedding_86": 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"title+abstract_embedding_109": -0.07768157, "title+abstract_embedding_110": 0.058832645, "title+abstract_embedding_111": 0.13968644, "title+abstract_embedding_112": -0.15538098, "title+abstract_embedding_113": -0.03988871, "title+abstract_embedding_114": 0.12578925, "title+abstract_embedding_115": -0.005558863, "title+abstract_embedding_116": -0.058881402, "title+abstract_embedding_117": -0.006885819, "title+abstract_embedding_118": -0.33986735, "title+abstract_embedding_119": 0.005258516, "title+abstract_embedding_120": 0.16521974, "title+abstract_embedding_121": -0.000652295, "title+abstract_embedding_122": -0.09290147, "title+abstract_embedding_123": 0.11907043, "title+abstract_embedding_124": -0.015804775, "title+abstract_embedding_125": -0.116001956, "title+abstract_embedding_126": -0.08598341, "title+abstract_embedding_127": 0.13814314, "label": 3, "label-multi": "1;3" }, { "paper_new_id": 48, "id": "j_3a0757ba2f3bb1a1129b1cafa59acf42", "title+abstract": "Pd-Ru-Bi nanoalloys modified three-dimensional reduced graphene oxide/MOF-199 composites as a highly efficient electrocatalyst for ethylene glycol electrooxidation;Abstract Well-dispersed trimetallic Pd-Ru-Bi alloy nanoparticles (NPs) were successfully embedded in the three-dimensional (3D) rGO/MOF-199 by a facile hydrothermal and in situ impregnation-reduction method. Among the mono-, bi- and tri-metal@rGO/MOF-199 electrocatalysts, the trimetallic PdRuBi@rGO/MOF-199 exhibited the highest catalytic activity and durability towards ethylene glycol oxidation reaction (EGOR) under the alkaline condition, as high as 213.93?mA?cm?2, is about 7.23 times higher than that of commercial Pd/C. The outstanding electrocatalysis oxidation performance of the PdRuBi@rGO/MOF-199 is attributed to the unique 3D structures with trimetallic composition and strong synergistic effects of Pd, Ru and Bi nanoalloys that providing plenty of interfaces and achievable reaction active sites. Furthermore, the introduction of GO in MOF-199 matrix conduces to the superior electron transfer and large surface area, which are beneficial to improve the catalytic ability of the catalyst. The study on the new composites offers a conception and applicable way to develop the advanced Pd-based electrocatalysts for high performance direct ethylene glycol fuel cells.", "title+abstract_embedding_0": 0.24598467, "title+abstract_embedding_1": -0.767792, "title+abstract_embedding_2": -0.3749533, "title+abstract_embedding_3": -0.58282006, "title+abstract_embedding_4": 0.29698914, "title+abstract_embedding_5": 0.47564936, "title+abstract_embedding_6": -0.49456432, "title+abstract_embedding_7": 0.24912007, "title+abstract_embedding_8": 0.1875992, "title+abstract_embedding_9": -0.027407348, "title+abstract_embedding_10": 0.000930756, "title+abstract_embedding_11": -0.08080538, "title+abstract_embedding_12": -0.07439482, "title+abstract_embedding_13": -0.042689614, "title+abstract_embedding_14": -0.020451173, "title+abstract_embedding_15": 0.25041935, "title+abstract_embedding_16": 0.07086265, "title+abstract_embedding_17": -0.23659481, "title+abstract_embedding_18": 0.19014387, 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"title+abstract_embedding_109": -0.063335866, "title+abstract_embedding_110": 0.12378782, "title+abstract_embedding_111": -0.018033883, "title+abstract_embedding_112": -0.051729128, "title+abstract_embedding_113": 0.01911489, "title+abstract_embedding_114": -0.22699985, "title+abstract_embedding_115": 0.036671244, "title+abstract_embedding_116": -0.01283104, "title+abstract_embedding_117": 0.05535825, "title+abstract_embedding_118": -0.19073339, "title+abstract_embedding_119": 0.07022469, "title+abstract_embedding_120": -0.01018139, "title+abstract_embedding_121": 0.07590484, "title+abstract_embedding_122": -0.05618748, "title+abstract_embedding_123": 0.13255215, "title+abstract_embedding_124": 0.11617111, "title+abstract_embedding_125": 0.06515515, "title+abstract_embedding_126": 0.030736864, "title+abstract_embedding_127": -0.050797537, "label": 3, "label-multi": "1;2;3" }, { "paper_new_id": 49, "id": "j_3a591dda3cde6c6df06d0203f22241d0", "title+abstract": "Highly active electrocatalysts of iron phthalocyanine by MOFs for oxygen reduction reaction under alkaline solution;Rational design of FePc and MOFs can result in good nanoarchitecture Fe¡§CN/C catalysts with improved ORR activity and stability.
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"title+abstract_embedding_114": -0.041633323, "title+abstract_embedding_115": 0.23859715, "title+abstract_embedding_116": -0.021304816, "title+abstract_embedding_117": -0.19545357, "title+abstract_embedding_118": -0.36073056, "title+abstract_embedding_119": -0.111760676, "title+abstract_embedding_120": 0.012761358, "title+abstract_embedding_121": -0.19256145, "title+abstract_embedding_122": 0.022884697, "title+abstract_embedding_123": 0.045903526, "title+abstract_embedding_124": -0.07851251, "title+abstract_embedding_125": -0.062276654, "title+abstract_embedding_126": 0.06912744, "title+abstract_embedding_127": -0.110956, "label": 3, "label-multi": "3" }, { "paper_new_id": 50, "id": "j_3a9518c203d613f24109121e4b4a86c4", "title+abstract": "Catalytic Kinetics || Heterogeneous Catalytic Kinetics;Basic kinetics schemes for heterogeneous catalytic reactions such as Eley-Rideal, Langmuir-Hinshelwood, and two-step sequence are considered. Examples of rate derivation for complex reactions with one route are presented. Kinetic models are presented for reactions on real surfaces with intrinsic or induced nonuniformity. Kinetics of single-route Christiansen sequences as well as consecutive and parallel reactions is discussed. Approaches are given for accounting of the multicentered nature of adsorbed compounds in kinetic modeling. Kinetic models where the solvent effects are incorporated in the rate equations beyond considerations of gas solubility and solvent adsorption are advanced. Kinetics of transfer of labeled atoms in heterogeneous catalytic reactions is illustrated with several examples. Electrocatalytic and photocatalytic kinetics is considered as special cases of heterogeneous catalytic kinetics. Cluster-size-dependent kinetics is quantitatively treated.", "title+abstract_embedding_0": -0.66451293, "title+abstract_embedding_1": -0.44586787, "title+abstract_embedding_2": 1.2361712, "title+abstract_embedding_3": -0.20516133, "title+abstract_embedding_4": -0.075715005, "title+abstract_embedding_5": 0.5671058, "title+abstract_embedding_6": -0.62482345, "title+abstract_embedding_7": 0.33848524, "title+abstract_embedding_8": 0.08316353, "title+abstract_embedding_9": 0.61576074, "title+abstract_embedding_10": 0.18664649, "title+abstract_embedding_11": -0.20893255, "title+abstract_embedding_12": 0.48002714, "title+abstract_embedding_13": -0.2460671, "title+abstract_embedding_14": 0.25320455, "title+abstract_embedding_15": 0.02875955, "title+abstract_embedding_16": 0.4932723, "title+abstract_embedding_17": -0.30026317, "title+abstract_embedding_18": -0.1225169, "title+abstract_embedding_19": -0.051155087, "title+abstract_embedding_20": -0.10813466, "title+abstract_embedding_21": 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"title+abstract_embedding_113": -0.006809235, "title+abstract_embedding_114": -0.083902664, "title+abstract_embedding_115": -0.0607607, "title+abstract_embedding_116": -0.041324407, "title+abstract_embedding_117": -0.030398428, "title+abstract_embedding_118": 0.23725863, "title+abstract_embedding_119": -0.039212752, "title+abstract_embedding_120": 0.001060011, "title+abstract_embedding_121": -0.10968232, "title+abstract_embedding_122": 0.14533502, "title+abstract_embedding_123": 0.1074745, "title+abstract_embedding_124": -0.021510385, "title+abstract_embedding_125": -0.023504466, "title+abstract_embedding_126": 0.012290444, "title+abstract_embedding_127": 0.18907006, "label": 106, "label-multi": NaN }, { "paper_new_id": 51, "id": "j_3cc73aa541c9819f8e42a08670cc6a54", "title+abstract": "Kinetic modeling for phenol degradation using photo-impinging streams reactor;In the present study, a novel kinetic model has been proposed for photocatalytic degradation of wastewater. In the first step, statistical experimental designs have been used to optimize the process of phenol degradation in a photo-impinging streams reactor. The crucial parameters, namely phenol concentration, catalyst loading, pH, and slurry flow rate, were selected for process optimization, applying central composite design. The analysis results indicated that interactions between catalyst loading and pH significantly affect phenol degradation. The predicted data showed that the maximum removal efficiency of phenol (99?%) could be obtained under the optimum operating conditions (phenol concentration?=?50?mg?l?1, catalyst loading?=?2.1?g?l?1, pH 6.2, and slurry flow rate?=?550?ml?min?1). These predicted values were then verified by certain validating experiments. Residence time distribution (RTD) of the slurry phase within the reactor was then measured using the impulse tracer method. A number of different assumptions were made, i.e., continuous stirred tank reactors (CSTRs) in series model and gamma distribution model with bypass (GDB). A comparison made between the sum of the square errors for experimental and predicted RTD values in case of each flow model revealed that both CSTRs in series model and GDB were proper descriptions for reactor behavior. The CSTRs in series model and RTD data were applied in conjunction with the phenol degradation kinetic model to predict the coefficients of the reaction rate.", "title+abstract_embedding_0": 0.35267532, "title+abstract_embedding_1": -0.07148832, "title+abstract_embedding_2": 1.8369814, "title+abstract_embedding_3": 0.6989174, "title+abstract_embedding_4": -0.03925395, "title+abstract_embedding_5": -0.30071646, "title+abstract_embedding_6": -0.31235734, "title+abstract_embedding_7": -0.26257595, "title+abstract_embedding_8": 0.3681533, "title+abstract_embedding_9": 0.30762744, "title+abstract_embedding_10": -0.6550608, "title+abstract_embedding_11": -0.29943654, "title+abstract_embedding_12": -0.06676379, "title+abstract_embedding_13": -0.18894422, "title+abstract_embedding_14": 0.19778913, "title+abstract_embedding_15": 0.40013817, "title+abstract_embedding_16": 0.38576645, "title+abstract_embedding_17": -0.66900253, "title+abstract_embedding_18": -0.035917334, 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"title+abstract_embedding_109": -0.022812307, "title+abstract_embedding_110": -0.10771337, "title+abstract_embedding_111": 0.000225496, "title+abstract_embedding_112": 0.06941362, "title+abstract_embedding_113": -0.08420341, "title+abstract_embedding_114": -0.030277833, "title+abstract_embedding_115": 0.115402564, "title+abstract_embedding_116": 0.096193545, "title+abstract_embedding_117": 0.061331667, "title+abstract_embedding_118": -0.01206416, "title+abstract_embedding_119": -0.01745945, "title+abstract_embedding_120": -0.002017133, "title+abstract_embedding_121": -0.06711127, "title+abstract_embedding_122": 0.056911334, "title+abstract_embedding_123": -0.056855842, "title+abstract_embedding_124": -0.070861764, "title+abstract_embedding_125": -0.07848098, "title+abstract_embedding_126": -0.05688133, "title+abstract_embedding_127": 0.1056543, "label": 3, "label-multi": "3" }, { "paper_new_id": 52, "id": "j_3d4a4cc2c7206196aa044c52ca4f234b", "title+abstract": "One-pot synthesis of high-density Pd nanoflowers decorated 3D carbon nanotube-graphene network modified on printed electrode as portable electrochemical sensing platform for sensitive detection of nitroaromatic explosives;The maintenance of public security from warfare agents stimulates the growing demand in the development of portable sensors for explosives detection. In this work, a portable electrochemical sensor integrated with a nanohybrid modified printed electrode and miniaturized electrochemical readout, has been established for highly sensitive and rapid in situ detection of explosives. For the preparation of the modified printed electrode, the active electrode material Pd nanoflowers (PdNFs) decorated carbon nanotubes (CNTs)-graphene nanosheets (GNSs) nanocomposite (PdNFs-CNTs-GNSs) has been synthesized by a facile and effective one-pot chemical reduction and assembly from a mixture of their precursors, this enables the formation of highly dense and well dispersed PdNFs on 3D porous CNTs-GNSs network, which effectively increases the electrode active surface area and improves the electrocatalytic activity. For electrochemical detection of a series of explosive nitroaromatic compounds such as p-nitrophenol (4-NP), dinitrobenzene (DNB), 1-choloro-2,4-dinitrobenzene (Cl-DNB), 2,4-dinitrotoluene (DNT), trinitrobenzene (TNB) and trinitrotoluene (TNT), the developed portable electrochemical sensor with PdNFs-CNTs-GNSs modified printed electrode shows attractive analytical features such as good sensitivity, widely operational linear range for determination, low detection limit and high selectivity, and can be used for the sensitive and accurate measurement of nitroaromatic compounds in environmental samples.", "title+abstract_embedding_0": -0.020760536, "title+abstract_embedding_1": -1.004909, "title+abstract_embedding_2": -1.0703375, "title+abstract_embedding_3": 0.19257718, "title+abstract_embedding_4": -0.69873863, "title+abstract_embedding_5": -0.14156902, "title+abstract_embedding_6": -0.9939561, "title+abstract_embedding_7": 0.43656188, "title+abstract_embedding_8": -0.38999224, 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"title+abstract_embedding_122": -0.09605634, "title+abstract_embedding_123": -0.07810653, "title+abstract_embedding_124": 0.040020227, "title+abstract_embedding_125": 0.047308415, "title+abstract_embedding_126": -0.051523305, "title+abstract_embedding_127": -0.10752082, "label": 3, "label-multi": "14;3" }, { "paper_new_id": 53, "id": "j_3ddd43423a3cf836c5ce8aeb29aae2d9", "title+abstract": "Phosphate group grafted twinned BiPO4 with significantly enhanced photocatalytic activity: Synergistic effect of improved charge separation efficiency and redox ability;The photocatalytic technology based on solar energy is a potential approach to mitigate environmental problem. The surface property of photocatalysts and the separation efficiency of photo-generated spatial charge are considerably important to enhance their photocatalytic activity in the decomposition of organic pollutants in wastewater. In this work, phosphate group grafted twinned BiPO4 with surface phase junction were controllably synthesized by a facile two-step method. XRD results showed that two crystal phases of nMBIP and mMBIP were formed in the twinned BiPO4. The formation of phase junction in BiPO4 was also validated by HRTEM. XPS spectra confirmed that PO43- successfully grafted on the surface of the twinned BiPO4. The apparent rate constants of the twinned BiPO4 for degradation of methylene blue (MB) and carbamazepine (CBZ) improved 5.3 and 5.0 times respectively compared to pristine BiPO4 because of the formed phase junction. After phosphate grafting on the surface of phase junction, the apparent rate constants for MB and CBZ degradation were further boosted, which were 3.0 and 5.2 times as high as that of twinned BiPO4. The photocatalytic intermediates of CBZ were detected by HPLC-ESI-MS/MS, and a deductive degradation pathway of CBZ was proposed. Transient photocurrent responses, PL and Mott-Schottky analysis verified that the enhanced photocatalytic activity of phosphate group grafted twinned BiPO4 with phase junction for the degradation of MB and CBZ was ascribed to faster transfer, efficient separation and improved redox ability of photo-induced charge carriers.", "title+abstract_embedding_0": 1.2096444, "title+abstract_embedding_1": 0.55836046, "title+abstract_embedding_2": 0.17212823, "title+abstract_embedding_3": -0.41337705, "title+abstract_embedding_4": -0.4029831, "title+abstract_embedding_5": -0.28481513, "title+abstract_embedding_6": 0.009534895, "title+abstract_embedding_7": 0.04187336, "title+abstract_embedding_8": -0.36201397, "title+abstract_embedding_9": 0.2698076, "title+abstract_embedding_10": 0.1344037, "title+abstract_embedding_11": -0.20968649, "title+abstract_embedding_12": 0.07607485, "title+abstract_embedding_13": -0.2103037, "title+abstract_embedding_14": -0.095290914, "title+abstract_embedding_15": 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-0.08061108, "label": 3, "label-multi": "0;3" }, { "paper_new_id": 54, "id": "j_3de62a9050d748ec50e31e9711653dee", "title+abstract": "Direct synthesis of nano titania on highly-ordered mesoporous SBA-15 framework for enhancing adsorption and photocatalytic activity;This paper reports the synthesis of TiO2-containing mesoporous catalysts for effectively enhancing the adsorption and photocatalytic activity. The factors that affect the photocatalytic activity of catalyst composites, including types of silica support, TiO2 content, calcination temperature, and catalyst mass, were examined in this study. The samples were characterized by X-ray diffraction, field-emission scanning electron microscopy, transmission electron microscopy, thermogravimetric analysis, and surface area analysis. The experimental results showed that incorporating TiO2 nanoparticles into silica gel or SBA-15 frameworks could enhance the photodegradation rate more effectively than pure TiO2. The TiO2/SBA-15 sample displayed much higher adsorption and photocatalytic activity levels than did TiO2/silica-gel. The pore volume and pore size of TiO2/SBA-15 were as high as 1.317?cm3/g and 7.51?nm, respectively, which exceeded those of TiO2/silica-gel (0.437?cm3/g and 3.68?nm, respectively). The rate constants of photocatalysis were determined. The photodegradation rate of the catalyst increased with decreasing TiO2 content and increasing calcination temperature. The proposed method of preparing mesoporous photocatalysts is simple and suitable for mass production.", "title+abstract_embedding_0": 0.9464046, "title+abstract_embedding_1": 0.63849473, "title+abstract_embedding_2": -0.0758197, "title+abstract_embedding_3": 0.43875182, "title+abstract_embedding_4": 0.85245806, "title+abstract_embedding_5": 0.67318153, "title+abstract_embedding_6": -0.3592702, "title+abstract_embedding_7": 0.02434133, "title+abstract_embedding_8": -0.002267358, "title+abstract_embedding_9": 0.21370363, "title+abstract_embedding_10": 0.105720446, "title+abstract_embedding_11": 0.001499519, "title+abstract_embedding_12": -0.12509465, "title+abstract_embedding_13": 0.14614892, "title+abstract_embedding_14": -0.10042426, "title+abstract_embedding_15": -0.000955853, "title+abstract_embedding_16": 0.29316807, "title+abstract_embedding_17": -0.04421577, "title+abstract_embedding_18": -0.2706042, "title+abstract_embedding_19": -0.113289475, "title+abstract_embedding_20": 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"title+abstract_embedding_110": 0.18999279, "title+abstract_embedding_111": 0.09361444, "title+abstract_embedding_112": -0.028551951, "title+abstract_embedding_113": 0.07355237, "title+abstract_embedding_114": 0.056249008, "title+abstract_embedding_115": 0.026784934, "title+abstract_embedding_116": 0.02126253, "title+abstract_embedding_117": -0.06477931, "title+abstract_embedding_118": -0.097526185, "title+abstract_embedding_119": 0.023034038, "title+abstract_embedding_120": -0.058511578, "title+abstract_embedding_121": 0.072920494, "title+abstract_embedding_122": -0.012058854, "title+abstract_embedding_123": 0.16898137, "title+abstract_embedding_124": 0.05855024, "title+abstract_embedding_125": 0.10190027, "title+abstract_embedding_126": -0.033354245, "title+abstract_embedding_127": 0.11291444, "label": 3, "label-multi": "1;3" }, { "paper_new_id": 55, "id": "j_3fae5c759f09cb3c46f44caa2957328d", "title+abstract": "Photochemistry and photocatalytic reactions of mixed-ligand azido transition metal complexes;Abstract Mechanistic details of the photolysis of mixed-ligand azido metal(II) complexes 1 (M = Pd(II), Pt(II), Ni(II); X-X = 2 PR 3 , R 2 P(CH 2 )nPR 2 , R-N=CH-CH=N-R ) are discussed with respect to formation of intermediate isomerization products, metal(I) complexes and azidyl radicals, respectively. Coordinatively unsaturated metal(O) complexes formed as the ultimate products in the course of photoreaction (1) exhibit catalytic activity. Thus, oxidative addition has been observed with photochemically generated platinum(O) and palladium(O) species whereas photoinduced cyclotrimerization of alkynes has been detected in the presence mixed-ligand azido nickel(II) complexes. cyclotrimerization of alkynes. Under similar aspects we have been able to prove the advantages of photocatalysis in oxygenation reactions of olefins in the presence of various metallo porphyrins 3,36¡§C38] and metal acetylacetonates [39], respectively. A more comprehensive review on homogeneous photocatalysis in organic synthesis is going to be published elsewhere [40].", "title+abstract_embedding_0": 0.29662764, "title+abstract_embedding_1": 0.83640504, "title+abstract_embedding_2": 0.56874126, "title+abstract_embedding_3": -1.0626075, "title+abstract_embedding_4": -0.29730904, "title+abstract_embedding_5": 0.20654255, "title+abstract_embedding_6": 0.006303638, "title+abstract_embedding_7": 0.90813744, "title+abstract_embedding_8": 0.03421851, "title+abstract_embedding_9": -0.18767148, "title+abstract_embedding_10": 0.64120764, "title+abstract_embedding_11": -0.17151581, "title+abstract_embedding_12": 0.4338568, "title+abstract_embedding_13": -0.19595832, "title+abstract_embedding_14": 0.3633851, "title+abstract_embedding_15": -0.2879437, "title+abstract_embedding_16": -0.48705196, "title+abstract_embedding_17": 0.33057162, "title+abstract_embedding_18": -0.056791082, "title+abstract_embedding_19": -0.08546479, 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"title+abstract_embedding_110": 0.006816298, "title+abstract_embedding_111": 0.03833811, "title+abstract_embedding_112": 0.035030648, "title+abstract_embedding_113": -0.10691236, "title+abstract_embedding_114": 0.04450059, "title+abstract_embedding_115": 0.007110298, "title+abstract_embedding_116": 0.10148276, "title+abstract_embedding_117": 0.077217646, "title+abstract_embedding_118": -0.02237115, "title+abstract_embedding_119": 0.0343508, "title+abstract_embedding_120": 0.05921724, "title+abstract_embedding_121": -0.048752762, "title+abstract_embedding_122": 0.055128768, "title+abstract_embedding_123": 0.27577707, "title+abstract_embedding_124": -0.02514077, "title+abstract_embedding_125": -0.014440127, "title+abstract_embedding_126": 0.04445465, "title+abstract_embedding_127": 0.09389569, "label": 3, "label-multi": "3" }, { "paper_new_id": 56, "id": "j_4053540c7067882a4a4bfd0917465bed", "title+abstract": "Photodegradation of Famotidine by Integrated Photocatalytic Adsorbent (IPCA) and Kinetic Study;Integrated photocatalytic adsorbents (IPCAs) comprised of nanocrystalline titanium dioxide (TiO2) and activated carbon (AC) were prepared using an ultrasonic impregnation technique. The IPCAs were characterised by scanning electron microscopy (SEM) and Fourier-transform infrared (FT-IR) spectroscopy and were employed as catalysts for the photodegradation of famotidine-an active pharmaceutical ingredient-in aqueous solutions using illumination from a 125?W medium pressure mercury lamp. The degradation kinetics were found to follow a pseudo-first-order rate law and varying TiO2 loadings induced different increases in the apparent first-order rate constant of the process. The kinetic behaviour can be described in terms of a modified Langmuir¡§CHinshelwood (LH) model. The IPCA prepared using a 10% TiO2 to AC loading exhibited the highest rate constant with a KC and kr of 0.0172 L/mg and 0.237?mg/L/min, respectively. The LH model fits the experimental data and elucidates the effect of the TiO2 content of the IPCA on the degradation rate. The use of calcination (heat treatment) in IPCA preparation and its effect on photocatalytic and adsorption performance were also investigated. The present work demonstrates that the combination of TiO2 and AC results in a promising material for application in the degradation of organic pollutants.Graphical AbstractThe values of the adsorption equilibrium constants, KC, and the rate constants, kr, for the photodegradation of famotidine were dependent on TiO2 content of IPCAs.", "title+abstract_embedding_0": 0.62125635, "title+abstract_embedding_1": 0.004235834, "title+abstract_embedding_2": 0.74885684, "title+abstract_embedding_3": 0.6393115, "title+abstract_embedding_4": 0.18992883, "title+abstract_embedding_5": -0.0445773, "title+abstract_embedding_6": -0.43512455, "title+abstract_embedding_7": -0.0744655, "title+abstract_embedding_8": -0.002549446, "title+abstract_embedding_9": -0.02273655, "title+abstract_embedding_10": -0.05866802, "title+abstract_embedding_11": -0.006125845, "title+abstract_embedding_12": 0.054933816, "title+abstract_embedding_13": 0.30838665, "title+abstract_embedding_14": 0.13826138, 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"title+abstract_embedding_105": 0.02834277, "title+abstract_embedding_106": 0.05821558, "title+abstract_embedding_107": 0.17911613, "title+abstract_embedding_108": 0.034056664, "title+abstract_embedding_109": 0.003299281, "title+abstract_embedding_110": -0.086877525, "title+abstract_embedding_111": -0.015345996, "title+abstract_embedding_112": 0.03445925, "title+abstract_embedding_113": 0.03476035, "title+abstract_embedding_114": 0.07498889, "title+abstract_embedding_115": -0.025952108, "title+abstract_embedding_116": 0.021318674, "title+abstract_embedding_117": -0.07125653, "title+abstract_embedding_118": -0.09792161, "title+abstract_embedding_119": -0.041201763, "title+abstract_embedding_120": -0.08102618, "title+abstract_embedding_121": 0.041199744, "title+abstract_embedding_122": 0.06961788, "title+abstract_embedding_123": -0.040992986, "title+abstract_embedding_124": -0.14358798, "title+abstract_embedding_125": -0.16314122, "title+abstract_embedding_126": -0.081770055, "title+abstract_embedding_127": -0.011846677, "label": 3, "label-multi": "3" }, { "paper_new_id": 57, "id": "j_41e2bf7b677a62d0e932db895f750104", "title+abstract": "Bimetallic PtAu alloy nanomaterials for nonenzymatic selective glucose sensing at low potential;Electrochemical nonenzymatic glucose sensing meets the challenge of excellent selectivity and the minimum poisoning effect of the electrode. Bimetallic alloys based on Pt have distinct synergistic characteristics and offer remarkable anti-poisoning capability and electrocatalytic performance for sensitive and selective glucose sensing at low potential. Bimetallic PtAu alloy nanomaterials loaded into nanocarbon carrier (PtAu/C) were successfully fabricated. The morphology and structure of PtAu bimetallic alloy were observed. The voltammetric response of the PtAu/C modified electrodes towards glucose oxidation in NaOH revealed significant enhanced compared with Pt/C or Au/C. PtAu (1:1)/C with 0.4 wt% content of Pt was used for selective glucose detection at a low potential of -0.33 V (vs. SCE). Interfering substances revealed inert and ignorable analytical influence on glucose detection. Furthermore, DPV was applied for sensitive determination of glucose. A linear relationship was found between peak current and glucose concentration within the range of 0.01-10 mM with the limit of detection (LOD) of 3 mu M. Validation in human serum samples indicated that the PtAu (1:1)/C (0.4 wt% Pt) modified electrode accurately detected glucose. The PtAu bimetallic alloy exhibited a bright prospect for the glucose analysis of real samples. (C) 2020 Elsevier B.V. All rights reserved.", "title+abstract_embedding_0": 0.39350152, "title+abstract_embedding_1": -1.2347465, "title+abstract_embedding_2": -0.35655192, "title+abstract_embedding_3": 0.68200964, "title+abstract_embedding_4": -0.32892436, "title+abstract_embedding_5": 0.18195996, "title+abstract_embedding_6": 0.33397606, "title+abstract_embedding_7": 0.025807165, "title+abstract_embedding_8": -0.20959146, "title+abstract_embedding_9": -0.2909543, "title+abstract_embedding_10": 0.2681146, "title+abstract_embedding_11": 0.54365265, "title+abstract_embedding_12": 0.23932748, "title+abstract_embedding_13": -0.20447254, "title+abstract_embedding_14": -0.635497, "title+abstract_embedding_15": 0.4048155, "title+abstract_embedding_16": -0.04033965, "title+abstract_embedding_17": 0.3875285, "title+abstract_embedding_18": 0.46104085, "title+abstract_embedding_19": -0.35024816, "title+abstract_embedding_20": 0.21654792, "title+abstract_embedding_21": 0.31371725, "title+abstract_embedding_22": 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"title+abstract_embedding_90": -0.22964802, "title+abstract_embedding_91": -0.066729434, "title+abstract_embedding_92": -0.23574649, "title+abstract_embedding_93": 0.21872672, "title+abstract_embedding_94": -0.063997135, "title+abstract_embedding_95": 0.25202772, "title+abstract_embedding_96": 0.073218465, "title+abstract_embedding_97": 0.005167685, "title+abstract_embedding_98": 0.0363478, "title+abstract_embedding_99": 0.13666129, "title+abstract_embedding_100": -0.18438196, "title+abstract_embedding_101": -0.10324603, "title+abstract_embedding_102": -0.036543153, "title+abstract_embedding_103": -0.12941155, "title+abstract_embedding_104": -0.099567115, "title+abstract_embedding_105": -0.06995103, "title+abstract_embedding_106": -0.022452146, "title+abstract_embedding_107": 0.1829695, "title+abstract_embedding_108": -0.17577216, "title+abstract_embedding_109": -0.12674038, "title+abstract_embedding_110": -0.08947432, "title+abstract_embedding_111": -0.110034026, "title+abstract_embedding_112": -0.064057276, "title+abstract_embedding_113": 0.022885628, "title+abstract_embedding_114": 0.26981384, "title+abstract_embedding_115": 0.13631593, "title+abstract_embedding_116": 0.16267426, "title+abstract_embedding_117": -0.088479176, "title+abstract_embedding_118": 0.11163089, "title+abstract_embedding_119": 0.11500767, "title+abstract_embedding_120": -0.16819301, "title+abstract_embedding_121": 0.1999784, "title+abstract_embedding_122": 0.006990939, "title+abstract_embedding_123": -0.007474691, "title+abstract_embedding_124": -0.008453541, "title+abstract_embedding_125": -0.12600368, "title+abstract_embedding_126": 0.0128485, "title+abstract_embedding_127": -0.13430086, "label": 3, "label-multi": "14;3" }, { "paper_new_id": 58, "id": "j_421c3e596739e13e87270de8c72f4abd", "title+abstract": "Au36(SPh)24 Nanomolecules: X-ray Crystal Structure, Optical Spectroscopy, Electrochemistry, and Theoretical Analysis;The physicochemical properties of gold:thiolate nanomolecules depend on their crystal structure and the capping ligands. The effects of protecting ligands on the crystal structure of the nanomolecules are of high interest in this area of research. Here we report the crystal structure of an all aromatic thiophenolate-capped Au36(SPh)24 nanomolecule, which has a face-centered cubic (fcc) core similar to other nanomolecules such as Au36(SPh-tBu)24 and Au36(SC5H9)24 with the same number of gold atoms and ligands. The results support the idea that a stable core remains intact even when the capping ligand is varied. We also correct our earlier assignment of \"Au36(SPh)23\" which was determined based on MALDI mass spectrometry which is more prone to fragmentation than ESI mass spectrometry. We show that ESI mass spectrometry gives the correct assignment of Au36(SPh)24, supporting the X-ray crystal structure. The electronic structure of the title compound was computed at different levels of theory (PBE, LDA, and LB94) using the coordinates extracted from the single crystal X-ray diffraction data. The optical and electrochemical properties were determined from experimental data using UV-vis spectroscopy, cyclic voltammetry, and differential pulse voltammetry. Au36(SPh)24 shows a broad electrochemical gap near 2 V, a desirable optical gap of ??1.75 eV for dye-sensitized solar cell applications, as well as appropriately positioned electrochemical potentials for many electrocatalytic reactions.", "title+abstract_embedding_0": 0.8169595, "title+abstract_embedding_1": -0.85659915, "title+abstract_embedding_2": -0.18070135, "title+abstract_embedding_3": -0.03748083, "title+abstract_embedding_4": -0.6582242, "title+abstract_embedding_5": 0.57765424, "title+abstract_embedding_6": 0.5884503, "title+abstract_embedding_7": 0.71074057, "title+abstract_embedding_8": 0.051136397, "title+abstract_embedding_9": -0.23585588, "title+abstract_embedding_10": 0.04021935, "title+abstract_embedding_11": 0.31996706, "title+abstract_embedding_12": 0.2762709, "title+abstract_embedding_13": 0.19672832, "title+abstract_embedding_14": 0.13844827, "title+abstract_embedding_15": -0.122605994, "title+abstract_embedding_16": -0.102234855, "title+abstract_embedding_17": 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"title+abstract_embedding_108": 0.1869858, "title+abstract_embedding_109": 0.11743887, "title+abstract_embedding_110": 0.086143196, "title+abstract_embedding_111": -0.14219595, "title+abstract_embedding_112": 0.058571145, "title+abstract_embedding_113": 0.070839435, "title+abstract_embedding_114": 0.07652585, "title+abstract_embedding_115": -0.06808325, "title+abstract_embedding_116": -0.042813145, "title+abstract_embedding_117": 0.13908786, "title+abstract_embedding_118": 0.06660809, "title+abstract_embedding_119": -0.01530479, "title+abstract_embedding_120": -0.020141246, "title+abstract_embedding_121": -0.061544694, "title+abstract_embedding_122": -0.027604401, "title+abstract_embedding_123": 0.12990281, "title+abstract_embedding_124": 0.097480126, "title+abstract_embedding_125": -0.04671455, "title+abstract_embedding_126": 0.117980614, "title+abstract_embedding_127": 0.05777736, "label": 3, "label-multi": "3" }, { "paper_new_id": 59, "id": "j_4573a1740fdac666e5082179d6afa751", "title+abstract": "Utilization of ecofriendly self-cleaning concrete using zinc oxide and polypropylene fibre;Abstract Self-cleaning concrete is also known as air purifying concrete. The main action of this concrete is to purify the indoor air pollutants inside the concrete and create ecofriendly environment. It is harmless to use and absorb the UV radiation reduce the harmful gases entering inside. Adding photocatalytic zinc oxide create an absorbent layer inside the concrete due to this formation we can reduce the smoke, harmful gases entraining agents. The approach of concrete is carried by the presence of sunlight to reduce air pollutants. Photo catalytic activity will not affect the nature of the concrete and its properties. In this study the strength of concrete is determined by photocatalyst zinc oxide and polypropylene fiber. The photocatalytic behavior is treated by coating indigo dye under UV exposure in concrete specimen.", "title+abstract_embedding_0": -0.46049708, "title+abstract_embedding_1": 0.617295, "title+abstract_embedding_2": 0.9057509, "title+abstract_embedding_3": 0.7260815, "title+abstract_embedding_4": -0.67662024, "title+abstract_embedding_5": 0.51696265, "title+abstract_embedding_6": -0.46626416, "title+abstract_embedding_7": -0.15182754, "title+abstract_embedding_8": 0.8181712, "title+abstract_embedding_9": 0.09427109, "title+abstract_embedding_10": -0.49984258, "title+abstract_embedding_11": 0.11094339, "title+abstract_embedding_12": 0.17160274, "title+abstract_embedding_13": 0.07893708, "title+abstract_embedding_14": 0.72898424, "title+abstract_embedding_15": 0.4930524, "title+abstract_embedding_16": -0.8864223, "title+abstract_embedding_17": -0.087604776, "title+abstract_embedding_18": -0.5021044, "title+abstract_embedding_19": 0.3733124, "title+abstract_embedding_20": 0.20973311, "title+abstract_embedding_21": 0.9621426, "title+abstract_embedding_22": -0.20171076, "title+abstract_embedding_23": 0.1196928, "title+abstract_embedding_24": 0.61203456, "title+abstract_embedding_25": 0.5831289, "title+abstract_embedding_26": 0.084527545, "title+abstract_embedding_27": 0.22805978, "title+abstract_embedding_28": -0.13140944, "title+abstract_embedding_29": -0.30484897, "title+abstract_embedding_30": 0.0644944, "title+abstract_embedding_31": 0.22314699, "title+abstract_embedding_32": 0.46977496, "title+abstract_embedding_33": 0.05088997, "title+abstract_embedding_34": 0.39805755, "title+abstract_embedding_35": -0.12577035, "title+abstract_embedding_36": -0.30405712, "title+abstract_embedding_37": -0.34699512, "title+abstract_embedding_38": 0.01313179, "title+abstract_embedding_39": 0.29025388, "title+abstract_embedding_40": 0.3144686, "title+abstract_embedding_41": 0.027065422, "title+abstract_embedding_42": -0.16557318, "title+abstract_embedding_43": -0.064690664, "title+abstract_embedding_44": -0.109266326, "title+abstract_embedding_45": -0.58629525, "title+abstract_embedding_46": -0.38562524, "title+abstract_embedding_47": -0.23521687, "title+abstract_embedding_48": 0.2327326, "title+abstract_embedding_49": 0.0284497, "title+abstract_embedding_50": -0.49074793, "title+abstract_embedding_51": -0.2794751, "title+abstract_embedding_52": 0.37576103, "title+abstract_embedding_53": 0.20762904, "title+abstract_embedding_54": -0.3097338, "title+abstract_embedding_55": 0.036056556, "title+abstract_embedding_56": -0.086556114, "title+abstract_embedding_57": -0.3942997, "title+abstract_embedding_58": -0.22906885, "title+abstract_embedding_59": -0.16198839, "title+abstract_embedding_60": -0.16461456, "title+abstract_embedding_61": -0.21981952, "title+abstract_embedding_62": 0.2631469, "title+abstract_embedding_63": -0.12754631, "title+abstract_embedding_64": -0.34507275, "title+abstract_embedding_65": -0.018449876, "title+abstract_embedding_66": 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"title+abstract_embedding_112": -0.2596292, "title+abstract_embedding_113": 0.13118038, "title+abstract_embedding_114": -0.007194668, "title+abstract_embedding_115": 0.083341785, "title+abstract_embedding_116": 0.18704344, "title+abstract_embedding_117": -0.04078415, "title+abstract_embedding_118": -0.20327935, "title+abstract_embedding_119": -0.18894137, "title+abstract_embedding_120": -0.26987153, "title+abstract_embedding_121": -0.21282704, "title+abstract_embedding_122": -0.22466275, "title+abstract_embedding_123": 0.1682477, "title+abstract_embedding_124": -0.12713736, "title+abstract_embedding_125": -0.24540353, "title+abstract_embedding_126": -0.10956223, "title+abstract_embedding_127": -0.19208455, "label": 106, "label-multi": NaN }, { "paper_new_id": 60, "id": "j_4746146d5b3ce773221ef4193c5027b6", "title+abstract": "Solar-hydrogen production with reduced graphene oxide supported CdxZn1-xS photocatalysts;Abstract Reduced graphene oxide (RGO)/CdxZn(1-x)S composites were firstly synthesized by thermal sulfurization method in one pot with elemental sulfur as sulfur source. By using one pot synthesis, CdxZn(1-x)S particles were decorated on the RGO sheets during sulfurization of Cd2+ and Zn2+ precursors. This synthesis method eased the control of the particle sizes of CdxZn(1-x)S by providing homogenous decoration of RGO with CdxZn(1-x)S particles and increased the strength between RGO sheet and CdxZn(1-x)S particles, which enhanced charge carrier mobility rate. Here, RGO in the composite structure supplied high electron conductivity, high adsorption capacity and extended light absorption ability. Thus, prepared RGO/CdxZn(1-x)S composites enhanced the photocatalytic activity. The crystal systems, lattice parameters, band gaps and surface morphologies of all photocatalysts are characterized to determine the factors that affected the photocatalytic activities of the composites. After that, the photocatalytic activities of prepared photocatalysts were tested by measuring H2 evolution rates. Among the composites, RGO/Cd0?¡è7Zn0?¡è3S structure possessed the highest H2 production rate (141.6 |¨¬molh?1) and apparent quantum efficiency (19.4%).", "title+abstract_embedding_0": 0.72891533, "title+abstract_embedding_1": 0.35970318, "title+abstract_embedding_2": -0.24557546, "title+abstract_embedding_3": -0.8961531, "title+abstract_embedding_4": -0.23266977, "title+abstract_embedding_5": -0.30714643, "title+abstract_embedding_6": 0.023236483, "title+abstract_embedding_7": -0.29556167, "title+abstract_embedding_8": 0.45520514, "title+abstract_embedding_9": -0.056952, "title+abstract_embedding_10": 0.19622523, "title+abstract_embedding_11": -0.30618787, "title+abstract_embedding_12": 0.031381667, "title+abstract_embedding_13": -0.46811816, "title+abstract_embedding_14": 0.044724017, "title+abstract_embedding_15": 0.102382995, "title+abstract_embedding_16": 0.16804922, "title+abstract_embedding_17": -0.028430626, "title+abstract_embedding_18": -0.21693307, "title+abstract_embedding_19": 0.19927947, "title+abstract_embedding_20": 0.2084452, "title+abstract_embedding_21": -0.34251165, "title+abstract_embedding_22": 0.103505984, "title+abstract_embedding_23": 0.0849691, "title+abstract_embedding_24": 0.17543201, "title+abstract_embedding_25": 0.052854717, "title+abstract_embedding_26": -0.20559728, "title+abstract_embedding_27": -0.07601829, "title+abstract_embedding_28": 0.4318192, "title+abstract_embedding_29": -0.024726398, "title+abstract_embedding_30": -0.050440505, "title+abstract_embedding_31": 0.059511207, "title+abstract_embedding_32": -0.06350597, "title+abstract_embedding_33": 0.15823925, "title+abstract_embedding_34": -0.12404916, "title+abstract_embedding_35": 0.2355178, "title+abstract_embedding_36": -0.21756256, "title+abstract_embedding_37": -0.17174412, "title+abstract_embedding_38": -0.080731854, "title+abstract_embedding_39": 0.115666084, "title+abstract_embedding_40": -0.11359918, "title+abstract_embedding_41": 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"title+abstract_embedding_87": -0.09739192, "title+abstract_embedding_88": 0.11045143, "title+abstract_embedding_89": -0.07584787, "title+abstract_embedding_90": -0.12587112, "title+abstract_embedding_91": 0.09646881, "title+abstract_embedding_92": -0.0207114, "title+abstract_embedding_93": 0.17389876, "title+abstract_embedding_94": -0.10555883, "title+abstract_embedding_95": 0.10611169, "title+abstract_embedding_96": 0.05592505, "title+abstract_embedding_97": -0.1208085, "title+abstract_embedding_98": 0.16599676, "title+abstract_embedding_99": 0.1663683, "title+abstract_embedding_100": 0.056242086, "title+abstract_embedding_101": -0.08554734, "title+abstract_embedding_102": -0.13936475, "title+abstract_embedding_103": -0.067565784, "title+abstract_embedding_104": -0.060657337, "title+abstract_embedding_105": 0.03992945, "title+abstract_embedding_106": -0.093494415, "title+abstract_embedding_107": -0.043683648, "title+abstract_embedding_108": -0.056891583, "title+abstract_embedding_109": -0.20338789, "title+abstract_embedding_110": 0.018898904, "title+abstract_embedding_111": 0.00462335, "title+abstract_embedding_112": 0.086971596, "title+abstract_embedding_113": -0.033495292, "title+abstract_embedding_114": 0.07593183, "title+abstract_embedding_115": -0.01821296, "title+abstract_embedding_116": 0.070749216, "title+abstract_embedding_117": -0.08562897, "title+abstract_embedding_118": 0.07251387, "title+abstract_embedding_119": -0.1638376, "title+abstract_embedding_120": -0.1320868, "title+abstract_embedding_121": -0.119072184, "title+abstract_embedding_122": -0.2131435, "title+abstract_embedding_123": 0.061030887, "title+abstract_embedding_124": 0.114356846, "title+abstract_embedding_125": -0.037257798, "title+abstract_embedding_126": 0.08778812, "title+abstract_embedding_127": 0.09537732, "label": 106, "label-multi": NaN }, { "paper_new_id": 61, "id": "j_47ea647a19389b9bc9f9e6876fe0ba8e", "title+abstract": "Photocatalytic properties of lanthanide tungstates Ln2W2O9 (Ln=La, Pr, Nd, Sm, and Gd);Abstract Lanthanide tungstates, Ln 2 W 2 O 9 (Ln=La, Pr, Nd, Sm, and Gd), were prepared via the polymerized complex method at 1273?K for 2?h, and their photocatalytic activities for hydrogen and oxygen evolution were investigated. Pt-loaded Gd 2 W 2 O 9 exhibited activity for H 2 evolution from an aqueous methanol solution under light irradiation ( |? >300?nm). The remaining Ln 2 W 2 O 9 were inactive for H 2 evolution due to the influence of the Ln elements and their crystal structures. All Ln 2 W 2 O 9 were inactive for O 2 evolution from an aqueous AgNO 3 solution due to the lack of O 2 evolution sites on the surface.", "title+abstract_embedding_0": 0.0938108, "title+abstract_embedding_1": 0.69717, "title+abstract_embedding_2": 0.8375473, "title+abstract_embedding_3": -0.54808307, "title+abstract_embedding_4": 0.35539895, "title+abstract_embedding_5": 0.25459397, "title+abstract_embedding_6": 1.0575312, "title+abstract_embedding_7": 0.110111475, "title+abstract_embedding_8": 0.09736645, "title+abstract_embedding_9": 0.07718685, "title+abstract_embedding_10": 0.21544248, "title+abstract_embedding_11": -0.055680193, "title+abstract_embedding_12": -0.17054415, "title+abstract_embedding_13": -0.22155994, "title+abstract_embedding_14": -0.10413666, "title+abstract_embedding_15": -0.040697664, "title+abstract_embedding_16": -0.10403474, "title+abstract_embedding_17": -0.305811, "title+abstract_embedding_18": 0.0116148, "title+abstract_embedding_19": 0.28908825, "title+abstract_embedding_20": -0.29808342, "title+abstract_embedding_21": -0.4845708, "title+abstract_embedding_22": -0.007383427, "title+abstract_embedding_23": -0.14700502, "title+abstract_embedding_24": -0.2243194, "title+abstract_embedding_25": -0.039748132, "title+abstract_embedding_26": -0.057071477, "title+abstract_embedding_27": -0.42795074, "title+abstract_embedding_28": 0.17475706, "title+abstract_embedding_29": 0.178725, "title+abstract_embedding_30": 0.079195976, "title+abstract_embedding_31": -0.15107091, "title+abstract_embedding_32": -0.15220907, "title+abstract_embedding_33": 0.17929102, "title+abstract_embedding_34": -0.08211291, "title+abstract_embedding_35": -0.047246754, "title+abstract_embedding_36": -0.44062293, "title+abstract_embedding_37": 0.1976238, "title+abstract_embedding_38": -0.06279248, "title+abstract_embedding_39": 0.11871708, "title+abstract_embedding_40": 0.45844877, "title+abstract_embedding_41": 0.02396786, "title+abstract_embedding_42": -0.13899274, "title+abstract_embedding_43": 0.01634024, "title+abstract_embedding_44": -0.23361175, "title+abstract_embedding_45": 0.23335922, "title+abstract_embedding_46": 0.074640065, "title+abstract_embedding_47": -0.05900104, "title+abstract_embedding_48": -0.005140215, "title+abstract_embedding_49": 0.5031109, "title+abstract_embedding_50": -0.35442787, "title+abstract_embedding_51": -0.19352776, "title+abstract_embedding_52": 0.39420694, "title+abstract_embedding_53": -0.06980313, "title+abstract_embedding_54": -0.23665917, "title+abstract_embedding_55": -0.13125518, "title+abstract_embedding_56": -0.022564705, "title+abstract_embedding_57": -0.051559612, "title+abstract_embedding_58": 0.02488415, "title+abstract_embedding_59": -0.29853427, "title+abstract_embedding_60": 0.061966434, "title+abstract_embedding_61": 0.11123511, "title+abstract_embedding_62": 0.29635945, "title+abstract_embedding_63": 0.07997471, "title+abstract_embedding_64": -0.1482558, "title+abstract_embedding_65": -0.3195619, "title+abstract_embedding_66": -0.40937847, "title+abstract_embedding_67": -0.0387522, "title+abstract_embedding_68": 0.16017003, "title+abstract_embedding_69": 0.20854461, "title+abstract_embedding_70": -0.037077434, "title+abstract_embedding_71": 0.055758968, "title+abstract_embedding_72": -0.16883668, "title+abstract_embedding_73": -0.165128, "title+abstract_embedding_74": 0.05312285, "title+abstract_embedding_75": 0.21039838, "title+abstract_embedding_76": -0.16991696, "title+abstract_embedding_77": 0.09828092, "title+abstract_embedding_78": -0.200313, "title+abstract_embedding_79": 0.16450812, "title+abstract_embedding_80": 0.10937992, "title+abstract_embedding_81": -0.363507, "title+abstract_embedding_82": -0.059435844, "title+abstract_embedding_83": -0.06497965, "title+abstract_embedding_84": 0.110808246, "title+abstract_embedding_85": -0.23536389, "title+abstract_embedding_86": -0.16217038, "title+abstract_embedding_87": -0.028099531, "title+abstract_embedding_88": 0.13309586, "title+abstract_embedding_89": 0.1196494, "title+abstract_embedding_90": -0.22482961, "title+abstract_embedding_91": 0.120028764, "title+abstract_embedding_92": 0.14604102, "title+abstract_embedding_93": 0.018232465, "title+abstract_embedding_94": 0.047417566, "title+abstract_embedding_95": -0.023433287, "title+abstract_embedding_96": 0.18057208, "title+abstract_embedding_97": -0.22463512, "title+abstract_embedding_98": 0.13900311, "title+abstract_embedding_99": -0.03883903, "title+abstract_embedding_100": -0.038124204, "title+abstract_embedding_101": 0.12309201, "title+abstract_embedding_102": 0.04816842, "title+abstract_embedding_103": 0.008821771, "title+abstract_embedding_104": -0.007879004, "title+abstract_embedding_105": -0.10292627, "title+abstract_embedding_106": -0.08336833, "title+abstract_embedding_107": -0.07137072, "title+abstract_embedding_108": 0.20957081, "title+abstract_embedding_109": 0.07296951, "title+abstract_embedding_110": 0.19238868, "title+abstract_embedding_111": 0.020601071, "title+abstract_embedding_112": -0.017925873, "title+abstract_embedding_113": -0.02842173, "title+abstract_embedding_114": -0.05444543, "title+abstract_embedding_115": -0.040212654, "title+abstract_embedding_116": 0.25271416, "title+abstract_embedding_117": -0.021923162, "title+abstract_embedding_118": 0.023860205, "title+abstract_embedding_119": 0.14941189, "title+abstract_embedding_120": 0.054229055, "title+abstract_embedding_121": -0.03376299, "title+abstract_embedding_122": -0.03798443, "title+abstract_embedding_123": 0.030584536, "title+abstract_embedding_124": 0.05872213, "title+abstract_embedding_125": 0.1721307, "title+abstract_embedding_126": -0.13321678, "title+abstract_embedding_127": -0.001760021, "label": 3, "label-multi": "2;3" }, { "paper_new_id": 62, "id": "j_48de6da6149664354f64eaea32dc6c6d", "title+abstract": "One-step synthesis of Zn doped titania nanotubes and investigation of their visible photocatalytic activity;Abstract Highly oriented undoped and Zn-doped titania (TiO2) nanotubes were electrochemically fabricated by one-step anodization of titanium foil in a freshly prepared aqueous solution of zinc fluoride (ZnF2) and ethylene glycol (EG). XRD and Raman spectroscopy unveiled the typical characteristic of anatase phase of TiO2 nanotube without any distinct dopant related peaks. SEM and AFM observation confirmed the formation of nanotubes and revealed that the Zn doping did not distort the tube morphology of TiO2. The doping of Zn was confirmed by energy dispersive X-ray as well as X-ray photospectroscopy. Due to one-step anodization process, instead of surface doping, the Zn2+ ions were incorporated into the bulk of TiO2 nanotubes. With increasing Zn doping in nanotubes, a gradual decrease in the band gap of TiO2 (2.84?eV) was observed. Photoluminescence measurements revealed that the doping of Zn enhanced the number of charge carriers, which eventually boosted the photocatalytic activity of TiO2 nanotubes. Compared to undoped nanotubes, the as prepared Zn-doped TiO2-nanotubes showed excellent photocatalytic activity for methylene blue degradation (reaction rate constant k?=?0.19?min?1) under visible light irradiation.", "title+abstract_embedding_0": 0.8970171, "title+abstract_embedding_1": 0.29725707, "title+abstract_embedding_2": -1.3498548, "title+abstract_embedding_3": 0.46119916, "title+abstract_embedding_4": 0.34467632, "title+abstract_embedding_5": -0.5034231, "title+abstract_embedding_6": 0.032761604, "title+abstract_embedding_7": 0.04641884, "title+abstract_embedding_8": -0.11011994, "title+abstract_embedding_9": 0.24493864, "title+abstract_embedding_10": 0.13465413, "title+abstract_embedding_11": -0.6746805, "title+abstract_embedding_12": 0.21964048, "title+abstract_embedding_13": -0.31429428, "title+abstract_embedding_14": 0.11591658, "title+abstract_embedding_15": -0.2846772, "title+abstract_embedding_16": -0.13248268, "title+abstract_embedding_17": 0.07945511, "title+abstract_embedding_18": 0.09558289, "title+abstract_embedding_19": 0.044743344, "title+abstract_embedding_20": -0.050554715, "title+abstract_embedding_21": -0.349303, "title+abstract_embedding_22": 0.054027088, "title+abstract_embedding_23": -0.11397773, "title+abstract_embedding_24": 0.014954358, "title+abstract_embedding_25": -0.3504506, "title+abstract_embedding_26": -0.3453996, "title+abstract_embedding_27": -0.08876313, "title+abstract_embedding_28": -0.17702019, "title+abstract_embedding_29": 0.038250487, "title+abstract_embedding_30": 0.14285955, "title+abstract_embedding_31": -0.04733073, "title+abstract_embedding_32": 0.23043263, "title+abstract_embedding_33": -0.08253795, "title+abstract_embedding_34": -0.27904955, "title+abstract_embedding_35": -0.16031188, "title+abstract_embedding_36": 0.29035512, "title+abstract_embedding_37": -0.28463018, "title+abstract_embedding_38": -0.029034749, "title+abstract_embedding_39": -0.004008725, "title+abstract_embedding_40": 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-0.027711362, "title+abstract_embedding_64": -0.032827094, "title+abstract_embedding_65": -0.031165864, "title+abstract_embedding_66": 0.004714388, "title+abstract_embedding_67": 0.06686306, "title+abstract_embedding_68": -0.07452114, "title+abstract_embedding_69": -0.09606269, "title+abstract_embedding_70": -0.04455132, "title+abstract_embedding_71": -0.07014115, "title+abstract_embedding_72": -0.099931404, "title+abstract_embedding_73": 0.013079235, "title+abstract_embedding_74": 0.25778317, "title+abstract_embedding_75": -0.07018524, "title+abstract_embedding_76": -0.03523621, "title+abstract_embedding_77": -0.054235205, "title+abstract_embedding_78": -0.04549127, "title+abstract_embedding_79": -0.19540685, "title+abstract_embedding_80": -0.013968352, "title+abstract_embedding_81": -0.26610234, "title+abstract_embedding_82": -0.039982796, "title+abstract_embedding_83": 0.11410793, "title+abstract_embedding_84": 0.005076006, "title+abstract_embedding_85": -0.000987507, "title+abstract_embedding_86": 0.018134568, "title+abstract_embedding_87": -0.084238574, "title+abstract_embedding_88": -0.120602965, "title+abstract_embedding_89": -0.08920381, "title+abstract_embedding_90": 0.119669944, "title+abstract_embedding_91": 0.12990882, "title+abstract_embedding_92": 0.047487408, "title+abstract_embedding_93": -0.030995227, "title+abstract_embedding_94": 0.06170936, "title+abstract_embedding_95": 0.023303505, "title+abstract_embedding_96": -0.060526736, "title+abstract_embedding_97": -0.002480668, "title+abstract_embedding_98": -0.08402321, "title+abstract_embedding_99": 0.15146902, "title+abstract_embedding_100": -0.04025072, "title+abstract_embedding_101": 0.060370013, "title+abstract_embedding_102": -0.07883118, "title+abstract_embedding_103": 0.03581579, "title+abstract_embedding_104": -0.055212677, "title+abstract_embedding_105": 0.007613078, "title+abstract_embedding_106": -0.071046785, "title+abstract_embedding_107": -0.039561465, "title+abstract_embedding_108": 0.05947885, "title+abstract_embedding_109": 0.078225926, "title+abstract_embedding_110": -0.057600945, "title+abstract_embedding_111": -0.050795943, "title+abstract_embedding_112": 0.03737046, "title+abstract_embedding_113": 0.17288576, "title+abstract_embedding_114": 0.0891124, "title+abstract_embedding_115": -0.07691886, "title+abstract_embedding_116": -0.017561488, "title+abstract_embedding_117": -0.011443891, "title+abstract_embedding_118": 0.055992715, "title+abstract_embedding_119": 0.12207365, "title+abstract_embedding_120": -0.22511186, "title+abstract_embedding_121": 0.13135332, "title+abstract_embedding_122": 0.021355003, "title+abstract_embedding_123": -0.06978686, "title+abstract_embedding_124": 0.13884123, "title+abstract_embedding_125": -0.01970791, "title+abstract_embedding_126": 0.0503807, "title+abstract_embedding_127": 0.04005059, "label": 106, "label-multi": NaN }, { "paper_new_id": 63, "id": "j_4a12d868d4dc307d347cf3748adfa9bb", "title+abstract": "TiO2 nanocrystallites photocatalysts modified with metallic species: Comparison between Cu and Pt doping;Abstract In this work, TiO2 nanoparticles were modified with different Cu and Pt species: metallic nanoparticles and ions. The photocatalysts were prepared via a sol-gel process by peptization with HNO3 at low temperature (i.e. 200 m2 g?1). The absorption property of these materials showed a visible sensitization for all samples even the pure TiO2 compared to the Evonik P25 due to N-doping confirmed by XPS analysis. The photocatalytic activity on the degradation of p-nitrophenol (PNP) showed an increase in the efficiency for nearly all catalysts compared to the pure one. Some mechanisms were proposed to explain these modifications of activity with doping. Under visible light, the photocatalysts were up to 5 times more efficient than P25 (for the best sample composed of Cu metallic nanoparticles).", "title+abstract_embedding_0": -0.002091885, "title+abstract_embedding_1": 1.2623299, "title+abstract_embedding_2": -0.322311, "title+abstract_embedding_3": 0.2600823, "title+abstract_embedding_4": 0.298971, "title+abstract_embedding_5": 0.436463, "title+abstract_embedding_6": 0.15601572, "title+abstract_embedding_7": -0.0468862, "title+abstract_embedding_8": 0.06540801, "title+abstract_embedding_9": 0.034128696, "title+abstract_embedding_10": 0.37780988, "title+abstract_embedding_11": 0.07416394, "title+abstract_embedding_12": 0.2954794, "title+abstract_embedding_13": -0.111473694, "title+abstract_embedding_14": 0.12376067, "title+abstract_embedding_15": 0.043183975, "title+abstract_embedding_16": 0.29932708, "title+abstract_embedding_17": -0.0297212, "title+abstract_embedding_18": -0.30076498, "title+abstract_embedding_19": -0.24780285, "title+abstract_embedding_20": -0.05331511, "title+abstract_embedding_21": 0.02069112, "title+abstract_embedding_22": 0.24531688, "title+abstract_embedding_23": 0.30324787, "title+abstract_embedding_24": -0.09680386, "title+abstract_embedding_25": 0.15341294, "title+abstract_embedding_26": 0.3178336, "title+abstract_embedding_27": 0.05528838, "title+abstract_embedding_28": -0.23820013, "title+abstract_embedding_29": 0.07895668, "title+abstract_embedding_30": -0.08256237, "title+abstract_embedding_31": -0.12428605, "title+abstract_embedding_32": 0.20042804, "title+abstract_embedding_33": -0.19012588, "title+abstract_embedding_34": 0.06052865, "title+abstract_embedding_35": 0.14073843, "title+abstract_embedding_36": 0.066726506, "title+abstract_embedding_37": -0.1339784, "title+abstract_embedding_38": 0.04405822, "title+abstract_embedding_39": 0.17369828, "title+abstract_embedding_40": 0.05251178, "title+abstract_embedding_41": 0.059486803, "title+abstract_embedding_42": 0.116939306, "title+abstract_embedding_43": -0.21609004, "title+abstract_embedding_44": -0.016725123, "title+abstract_embedding_45": 0.21083361, "title+abstract_embedding_46": -0.07232517, "title+abstract_embedding_47": 0.06285085, "title+abstract_embedding_48": -0.056060188, "title+abstract_embedding_49": 0.031120151, "title+abstract_embedding_50": -0.04935524, "title+abstract_embedding_51": -0.167009, "title+abstract_embedding_52": 0.1241394, "title+abstract_embedding_53": 0.03244468, "title+abstract_embedding_54": -0.022097215, "title+abstract_embedding_55": -0.06428982, "title+abstract_embedding_56": -0.025455486, "title+abstract_embedding_57": 0.19170037, "title+abstract_embedding_58": -0.15677729, "title+abstract_embedding_59": 0.11595503, "title+abstract_embedding_60": 0.028247356, "title+abstract_embedding_61": -0.026334114, "title+abstract_embedding_62": -0.09296351, "title+abstract_embedding_63": -0.12818211, "title+abstract_embedding_64": -0.040645808, "title+abstract_embedding_65": 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"title+abstract_embedding_88": -0.09443492, "title+abstract_embedding_89": 0.12124252, "title+abstract_embedding_90": 0.13487868, "title+abstract_embedding_91": 0.001356568, "title+abstract_embedding_92": 0.000519924, "title+abstract_embedding_93": 0.072918944, "title+abstract_embedding_94": 0.00397221, "title+abstract_embedding_95": 0.13223445, "title+abstract_embedding_96": -0.10905539, "title+abstract_embedding_97": -0.014708363, "title+abstract_embedding_98": -0.061500978, "title+abstract_embedding_99": -0.03388887, "title+abstract_embedding_100": -0.061132222, "title+abstract_embedding_101": 0.003452644, "title+abstract_embedding_102": 0.060911343, "title+abstract_embedding_103": -0.044212103, "title+abstract_embedding_104": 0.109840244, "title+abstract_embedding_105": 0.047814075, "title+abstract_embedding_106": 0.07138784, "title+abstract_embedding_107": -0.062982574, "title+abstract_embedding_108": 0.119341195, "title+abstract_embedding_109": -0.038078636, "title+abstract_embedding_110": 0.014737874, "title+abstract_embedding_111": -0.009253355, "title+abstract_embedding_112": -0.057913825, "title+abstract_embedding_113": -0.003464967, "title+abstract_embedding_114": -0.109705806, "title+abstract_embedding_115": 0.003824465, "title+abstract_embedding_116": -0.000226825, "title+abstract_embedding_117": -0.005384848, "title+abstract_embedding_118": -0.03916345, "title+abstract_embedding_119": 0.11278777, "title+abstract_embedding_120": -0.009236304, "title+abstract_embedding_121": -0.011506556, "title+abstract_embedding_122": 0.05733727, "title+abstract_embedding_123": 0.03535174, "title+abstract_embedding_124": 0.08503336, "title+abstract_embedding_125": 0.06329587, "title+abstract_embedding_126": 0.0708383, "title+abstract_embedding_127": -0.15133715, "label": 3, "label-multi": "1;2;3" }, { "paper_new_id": 64, "id": "j_4a72b870e543c847c3d772ce65f4847c", "title+abstract": "Gas chromatographic separation of PCB and OCP by photocatalytic degradation;Abstract A photocatalytic degradation method was developed for polychlorobiphenyl (PCB) and organochloride pesticide (OCP) discrimination and quantification. A mixture of Aroclor 1260 and p , p ??-DDT was irradiated at 254?nm by UV lamp (40?W) in the presence of TiO 2 (30?mg?mL ?1 non-aqueous solution). Comparison of gas chromatograms showed that p , p ??-DDT signals decreased significantly after irradiation, while Aroclor 1260s chromatograms did not show any difference before and after irradiation. Detection limits were 0.30?mg?L ?1 and 0.15?mg?L ?1 for p , p ??-DDT and Aroclor 1260, respectively. The method was applied to spiked egg samples, the recoveries were found as 72% for DDT and 82.01% for Aroclor 1260.", "title+abstract_embedding_0": 0.23040044, "title+abstract_embedding_1": 0.45229536, "title+abstract_embedding_2": 1.6116047, "title+abstract_embedding_3": 0.75205564, "title+abstract_embedding_4": -0.5153086, "title+abstract_embedding_5": -0.05459404, "title+abstract_embedding_6": 0.24971499, "title+abstract_embedding_7": 0.177683, "title+abstract_embedding_8": 0.23482208, "title+abstract_embedding_9": -0.2202335, "title+abstract_embedding_10": -0.108883426, "title+abstract_embedding_11": -0.006163381, "title+abstract_embedding_12": -0.29057094, "title+abstract_embedding_13": 0.03751839, "title+abstract_embedding_14": -0.123919785, "title+abstract_embedding_15": -0.067068845, "title+abstract_embedding_16": 0.33686882, "title+abstract_embedding_17": 0.091184825, "title+abstract_embedding_18": 0.026079297, "title+abstract_embedding_19": -0.10180564, 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0.11361271, "title+abstract_embedding_111": -0.17834884, "title+abstract_embedding_112": 0.04101385, "title+abstract_embedding_113": -0.19969194, "title+abstract_embedding_114": -0.15136859, "title+abstract_embedding_115": -0.22832423, "title+abstract_embedding_116": 0.24900001, "title+abstract_embedding_117": 0.14997292, "title+abstract_embedding_118": 0.024000164, "title+abstract_embedding_119": 0.06377095, "title+abstract_embedding_120": 0.04371695, "title+abstract_embedding_121": -0.0372874, "title+abstract_embedding_122": 0.12514909, "title+abstract_embedding_123": -0.07128849, "title+abstract_embedding_124": 0.060778808, "title+abstract_embedding_125": -0.096665375, "title+abstract_embedding_126": -0.00156711, "title+abstract_embedding_127": 0.05219073, "label": 3, "label-multi": "3" }, { "paper_new_id": 65, "id": "j_4ab176728262f44991e980688ac21f7e", "title+abstract": "Au-MoS2 Hybrids as Hydrogen Evolution Electrocatalysts;Core¡§Cshell nanoparticles provide a unique morphology to exploit electronic interactions between dissimilar materials, conferring upon them new or improved functionalities. MoS2 is a layered transition-metal disulfide that has been studied extensively for the hydrogen evolution reaction (HER) but still suffers from low electrocatalytic activity due to its poor electronic conductivity. To understand the fundamental aspects of the MoS2¡§CAu hybrids with regard to their electrocatalytic activity, a single to a few layers of MoS2 were deposited over Au nanoparticles via a versatile procedure that allows for complete encapsulation of Au nanoparticles of arbitrary geometries. High-resolution transmission electron microscopy of the Au@MoS2 nanoparticles provides direct evidence for the core¡§Cshell morphology and also reveals the presence of morphological defects and irregularities in the MoS2 shell that are known to be more active for HER than the pristine MoS2 basal plane. Electrochemical measurements show a signif...", "title+abstract_embedding_0": -0.20026457, "title+abstract_embedding_1": -0.87308973, "title+abstract_embedding_2": -0.5183542, "title+abstract_embedding_3": 0.12806684, "title+abstract_embedding_4": -0.04172814, "title+abstract_embedding_5": 0.5244438, "title+abstract_embedding_6": 0.6624515, "title+abstract_embedding_7": 0.08354734, "title+abstract_embedding_8": -0.13939188, "title+abstract_embedding_9": 0.5815705, "title+abstract_embedding_10": -0.059531912, "title+abstract_embedding_11": 0.51214796, "title+abstract_embedding_12": -0.31239942, "title+abstract_embedding_13": 0.40149817, "title+abstract_embedding_14": 0.01414898, "title+abstract_embedding_15": -0.67671865, "title+abstract_embedding_16": -0.21410242, "title+abstract_embedding_17": -0.47049066, "title+abstract_embedding_18": -0.44927692, "title+abstract_embedding_19": -0.02560855, "title+abstract_embedding_20": 0.2252448, "title+abstract_embedding_21": -0.54423296, 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"title+abstract_embedding_112": 0.17101169, "title+abstract_embedding_113": 0.013469942, "title+abstract_embedding_114": -0.09382633, "title+abstract_embedding_115": -0.055877067, "title+abstract_embedding_116": 0.023410782, "title+abstract_embedding_117": 0.09634169, "title+abstract_embedding_118": -0.047697566, "title+abstract_embedding_119": 0.14632809, "title+abstract_embedding_120": -0.092760384, "title+abstract_embedding_121": 0.10772625, "title+abstract_embedding_122": 0.030422807, "title+abstract_embedding_123": -0.17925581, "title+abstract_embedding_124": 0.012268409, "title+abstract_embedding_125": 0.017748602, "title+abstract_embedding_126": 0.09965177, "title+abstract_embedding_127": 0.09651204, "label": 3, "label-multi": "1;17;3" }, { "paper_new_id": 66, "id": "j_4cd29cc745ac59b7f4871ba9a6cf8593", "title+abstract": "The Role of Cobalt Phosphate in Enhancing the Photocatalytic Activity of ??¨¤-Fe2O3 toward Water Oxidation;Transient absorption spectroscopy was used to probe the dynamics of photogenerated charge carriers in |¨¢-Fe(2)O(3)/CoO(x) nanocomposite photoelectrodes for water splitting. The addition of cobalt-based electrocatalysts was observed to increase the lifetime of photogenerated holes in the photoelectrode by more than 3 orders of magnitude without the application of electrical bias. We therefore propose that the enhanced photoelectrochemical activity of the composite electrode for water photooxidation results, at least in part, from reduced recombination losses because of the formation of a Schottky-type heterojunction.", "title+abstract_embedding_0": -0.75841033, "title+abstract_embedding_1": 0.8970394, "title+abstract_embedding_2": -0.031753987, "title+abstract_embedding_3": -0.27766645, "title+abstract_embedding_4": -0.19718498, "title+abstract_embedding_5": -0.6178099, "title+abstract_embedding_6": 0.25193676, "title+abstract_embedding_7": -0.2992715, "title+abstract_embedding_8": -0.65230644, "title+abstract_embedding_9": -0.38268077, "title+abstract_embedding_10": -0.0513598, "title+abstract_embedding_11": -0.093294665, "title+abstract_embedding_12": -0.20301312, "title+abstract_embedding_13": 0.031038325, "title+abstract_embedding_14": 0.28722826, "title+abstract_embedding_15": -0.54173785, "title+abstract_embedding_16": 0.08168143, 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"title+abstract_embedding_108": -0.04855497, "title+abstract_embedding_109": -0.006914675, "title+abstract_embedding_110": -0.10597168, "title+abstract_embedding_111": -0.01322959, "title+abstract_embedding_112": -0.00134939, "title+abstract_embedding_113": -0.028134465, "title+abstract_embedding_114": 0.03794226, "title+abstract_embedding_115": 0.009750687, "title+abstract_embedding_116": 0.009549931, "title+abstract_embedding_117": -0.014883861, "title+abstract_embedding_118": 0.12522423, "title+abstract_embedding_119": -0.0989403, "title+abstract_embedding_120": -0.13403033, "title+abstract_embedding_121": 0.06861355, "title+abstract_embedding_122": -0.023281574, "title+abstract_embedding_123": 0.011508361, "title+abstract_embedding_124": 0.061885282, "title+abstract_embedding_125": -0.12336125, "title+abstract_embedding_126": 0.02647689, "title+abstract_embedding_127": -0.13740975, "label": 3, "label-multi": "3" }, { "paper_new_id": 67, "id": "j_4dafc5ce89ab71d101a68da80e4ccf00", "title+abstract": "A Pyrolysisa??Free Covalent Organic Polymer for Oxygen Reduction;Highly efficient electrocatalysts derived from metal¡§Corganic frameworks (MOFs) and covalent organic frameworks (COFs) for oxygen reduction reaction (ORR) have been developed. However, the subsequent pyrolysis is often needed owing to their poor intrinsic electrical conductivity, leading to undesirable structure changes and destruction of the original fine structure. Now, hybrid electrocatalysts were formed by self-assembling pristine covalent organic polymer (COP) with reduced graphene oxide (rGO). The electrical conductivity of the hybridized COP/rGO materials is increased by more than seven orders of magnitude (from 3.06?¨¢10?9 to 2.56?¨¢10?1 S m?1) compared with pure COPs. The ORR activities of the hybrid are enhanced significantly by the synergetic effect between highly active COP and highly conductive rGO. This COP/rGO hybrid catalyst exhibited a remarkable positive half-wave (150 mV).", "title+abstract_embedding_0": -0.7266848, "title+abstract_embedding_1": -0.89437217, "title+abstract_embedding_2": 0.49451414, "title+abstract_embedding_3": -0.48601985, "title+abstract_embedding_4": -0.15528321, "title+abstract_embedding_5": -0.19775885, "title+abstract_embedding_6": -0.26197037, "title+abstract_embedding_7": -0.20182207, "title+abstract_embedding_8": 0.1609703, "title+abstract_embedding_9": 0.25024083, "title+abstract_embedding_10": -0.2304464, "title+abstract_embedding_11": -0.2572261, "title+abstract_embedding_12": -0.3033063, "title+abstract_embedding_13": -0.1240677, "title+abstract_embedding_14": -0.1887435, "title+abstract_embedding_15": 0.105272084, "title+abstract_embedding_16": 0.114474356, "title+abstract_embedding_17": -0.14281392, "title+abstract_embedding_18": 0.36606294, "title+abstract_embedding_19": -0.095091596, "title+abstract_embedding_20": 0.20288871, 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"title+abstract_embedding_111": 0.09614367, "title+abstract_embedding_112": 0.042141512, "title+abstract_embedding_113": -0.275029, "title+abstract_embedding_114": 0.08151837, "title+abstract_embedding_115": -0.20636237, "title+abstract_embedding_116": -0.06768125, "title+abstract_embedding_117": 0.001124993, "title+abstract_embedding_118": -0.12533492, "title+abstract_embedding_119": -0.10498178, "title+abstract_embedding_120": -0.095507294, "title+abstract_embedding_121": -0.05739811, "title+abstract_embedding_122": 0.04180947, "title+abstract_embedding_123": 0.000625566, "title+abstract_embedding_124": -0.026474886, "title+abstract_embedding_125": 0.16314137, "title+abstract_embedding_126": 0.0541232, "title+abstract_embedding_127": 0.020691395, "label": 106, "label-multi": NaN }, { "paper_new_id": 68, "id": "j_4dcac557d7921c4c47e37dd510155473", "title+abstract": "Fabrication of layered (CdS-Mn/MoS2/CdTe)-promoted TiO2 nanotube arrays with superior photocatalytic properties;A novel (CdS-MniMoS(2)/CdTe)-sensitized TiO2 nanotube arrays (NTAs) photoelectrode has been prepared by electrodeposite, successive ionic layer adsorption and reaction (SILAR) coupled with hydrothermal method. When a ZnS layer was added on the top of CdS-Mn/MoS2/CdTe/TiO2, a notable red-shift and high absorption was observed in the visible light region. The photocurrent density (mA/cm(2)) systematically increases from TiO2 NTAs (0.43), CdTe/TiO2 (1.09), MoS2/CdTe/TiO2 (1.80), CdS-Mn/MoS2/CdTe/TiO2 (2.40), to ZnS/CdS-MniMoS(2)/CdTe/TiO2 (3.41) under visible light irradiation, due to the type-II semiconductor heterostructures comprising multiple components with a staggered band offset. Such a heterostructure possesses an enhanced photocatalytic performance towards degradation of organic contaminant, e.g. P-Nitrophenol (PNP) and Rhodamine B (RhB). (C) 2016 Elsevier Inc. All rights reserved.", "title+abstract_embedding_0": 0.7054163, "title+abstract_embedding_1": 0.4962337, "title+abstract_embedding_2": -0.70018566, "title+abstract_embedding_3": 0.1924591, "title+abstract_embedding_4": -0.041864276, "title+abstract_embedding_5": -0.30928946, "title+abstract_embedding_6": 0.5769042, "title+abstract_embedding_7": 0.19960208, "title+abstract_embedding_8": -0.106436275, "title+abstract_embedding_9": -0.18654096, "title+abstract_embedding_10": -0.12452093, "title+abstract_embedding_11": -0.5080451, "title+abstract_embedding_12": 0.1481444, "title+abstract_embedding_13": 0.08781595, "title+abstract_embedding_14": -0.30597943, "title+abstract_embedding_15": -0.03531963, "title+abstract_embedding_16": -0.11083609, "title+abstract_embedding_17": -0.17648153, "title+abstract_embedding_18": 0.14674215, "title+abstract_embedding_19": 0.23270099, "title+abstract_embedding_20": 0.058980152, "title+abstract_embedding_21": 0.33563617, "title+abstract_embedding_22": 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"title+abstract_embedding_112": 0.085999176, "title+abstract_embedding_113": -0.037324905, "title+abstract_embedding_114": 0.07799828, "title+abstract_embedding_115": 0.121362515, "title+abstract_embedding_116": -0.07251738, "title+abstract_embedding_117": 0.0722017, "title+abstract_embedding_118": 0.08589952, "title+abstract_embedding_119": -0.009712619, "title+abstract_embedding_120": 0.09212376, "title+abstract_embedding_121": 0.020068375, "title+abstract_embedding_122": -0.10895693, "title+abstract_embedding_123": 0.017029002, "title+abstract_embedding_124": 0.04069116, "title+abstract_embedding_125": 0.036385935, "title+abstract_embedding_126": -0.07065584, "title+abstract_embedding_127": -0.007237196, "label": 3, "label-multi": "3" }, { "paper_new_id": 69, "id": "j_4f57c84b60b264ede3ac2598a9ecc4af", "title+abstract": "Interfacing Plasmonic Nanoparticles with Ferroelectrics for Hot-Carrier-Driven Photocatalysis: Impact of Schottky Barrier Height;Emergent strategies for efficient solar energy conversion have focused on ways to harness photons in the lower-energy range of sunlight that cannot be utilized by conventional semiconductor photocatalyst systems. Recent research has demonstrated that interfaced plasmonic¡§Cferroelectric particles represent a promising strategy for the utilization of near-infrared (NIR) light owing to the possibility of the more?efficient injection of hot charge carriers from noble metal nanoparticles. Described herein, platinum-end-capped gold nanorods (AuNRs) function as antennae to absorb low-energy NIR photons to generate hot electrons that can be injected into ferroelectric PbZrxTi1¡§CxO3 (PZT; x = 0.48, 0.50, 0.52, 0.54, 0.56, and 0.60) and drive the reduction of water to molecular hydrogen at its surfaces. As an aqueous suspension, the interfaced AuNR-PZT particles exhibited maximal photocatalytic rates for hydrogen formation under a 976 nm diode laser (powder density = 2.0 W cm¡§C2) for the 52% Zr (x = 0.52) composition ...", "title+abstract_embedding_0": 0.22330296, "title+abstract_embedding_1": -0.017662048, "title+abstract_embedding_2": -0.74230576, "title+abstract_embedding_3": -0.53900623, "title+abstract_embedding_4": -0.38029796, "title+abstract_embedding_5": 0.39080232, "title+abstract_embedding_6": 0.6694284, "title+abstract_embedding_7": -0.49585393, "title+abstract_embedding_8": -0.05736118, "title+abstract_embedding_9": -0.7675718, "title+abstract_embedding_10": -0.16658923, "title+abstract_embedding_11": 0.21137184, "title+abstract_embedding_12": 0.13246873, "title+abstract_embedding_13": -0.17247841, "title+abstract_embedding_14": -0.13573518, "title+abstract_embedding_15": 0.022522908, "title+abstract_embedding_16": -0.121212915, "title+abstract_embedding_17": 0.27249113, 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"title+abstract_embedding_108": -0.044837505, "title+abstract_embedding_109": 0.009014741, "title+abstract_embedding_110": 0.12546441, "title+abstract_embedding_111": -0.047040693, "title+abstract_embedding_112": 0.07576303, "title+abstract_embedding_113": -0.06431569, "title+abstract_embedding_114": 0.13374868, "title+abstract_embedding_115": 0.028034873, "title+abstract_embedding_116": -0.051739343, "title+abstract_embedding_117": 0.067335166, "title+abstract_embedding_118": 0.09426336, "title+abstract_embedding_119": -0.09351961, "title+abstract_embedding_120": -0.12270683, "title+abstract_embedding_121": 0.077417895, "title+abstract_embedding_122": 0.06983371, "title+abstract_embedding_123": -0.044219993, "title+abstract_embedding_124": 0.00416062, "title+abstract_embedding_125": 0.053380072, "title+abstract_embedding_126": -0.031242846, "title+abstract_embedding_127": 0.15950239, "label": 3, "label-multi": "1;17;3" }, { "paper_new_id": 70, "id": "j_4f8b11f7b38f5bf5090f4e0fce4bf259", "title+abstract": "1D Coaxial Platinum/Titanium Nitride Nanotube Arrays with Enhanced Electrocatalytic Activity for the Oxygen Reduction Reaction: Towards Li-Air Batteries;CAT ON A HOT TIN SUPPORT: Coaxial Pt/TiN nanotube arrays are used to achieve a superior electrocatalytic activity of platinum towards the oxygen reduction reaction (ORR). Compared to a commercial Pt/C catalyst, the Pt/TiN?NTA materials delivers a higher mass activity and specific activity for the ORR. Hence, these materials are useful as cathodes for hybrid electrolyte Li-air batteries, as demonstrated.", "title+abstract_embedding_0": -1.721551, "title+abstract_embedding_1": -0.23548499, "title+abstract_embedding_2": -1.0218627, "title+abstract_embedding_3": 0.5829502, "title+abstract_embedding_4": 0.5969191, "title+abstract_embedding_5": 0.17017639, "title+abstract_embedding_6": -0.031998992, "title+abstract_embedding_7": 0.17476836, "title+abstract_embedding_8": 0.9044361, "title+abstract_embedding_9": -0.5828476, "title+abstract_embedding_10": -0.24842519, "title+abstract_embedding_11": 0.021919876, "title+abstract_embedding_12": 0.690634, "title+abstract_embedding_13": -0.017877713, "title+abstract_embedding_14": -0.630854, "title+abstract_embedding_15": -0.14234662, "title+abstract_embedding_16": -0.7794236, "title+abstract_embedding_17": 1.1666754, "title+abstract_embedding_18": 0.03129068, "title+abstract_embedding_19": -0.11980885, "title+abstract_embedding_20": -0.12742291, "title+abstract_embedding_21": 0.1953296, "title+abstract_embedding_22": -0.42206928, "title+abstract_embedding_23": 2.9414892e-05, "title+abstract_embedding_24": -0.30487302, "title+abstract_embedding_25": -0.08895475, "title+abstract_embedding_26": 0.42841575, "title+abstract_embedding_27": 0.15352722, "title+abstract_embedding_28": 0.34557045, "title+abstract_embedding_29": -0.30673316, "title+abstract_embedding_30": -0.16569059, "title+abstract_embedding_31": -0.006972415, "title+abstract_embedding_32": 0.31199023, "title+abstract_embedding_33": -0.11799723, "title+abstract_embedding_34": 0.36172372, "title+abstract_embedding_35": 0.015196554, "title+abstract_embedding_36": -0.019262418, "title+abstract_embedding_37": 0.033898845, "title+abstract_embedding_38": 0.48010394, "title+abstract_embedding_39": -0.007778192, "title+abstract_embedding_40": -0.17752063, "title+abstract_embedding_41": -0.05496682, "title+abstract_embedding_42": -0.39097235, "title+abstract_embedding_43": 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"title+abstract_embedding_66": 0.026495498, "title+abstract_embedding_67": 0.11803448, "title+abstract_embedding_68": 0.49924606, "title+abstract_embedding_69": 0.2714258, "title+abstract_embedding_70": 0.05824803, "title+abstract_embedding_71": 0.003363401, "title+abstract_embedding_72": -0.25122228, "title+abstract_embedding_73": -0.18613788, "title+abstract_embedding_74": 0.14943781, "title+abstract_embedding_75": 0.1412103, "title+abstract_embedding_76": -0.058264583, "title+abstract_embedding_77": 0.11553853, "title+abstract_embedding_78": 0.06955607, "title+abstract_embedding_79": -0.1696589, "title+abstract_embedding_80": 0.06042026, "title+abstract_embedding_81": 0.06309013, "title+abstract_embedding_82": 0.04481779, "title+abstract_embedding_83": -0.121109664, "title+abstract_embedding_84": 0.037541255, "title+abstract_embedding_85": -0.007964576, "title+abstract_embedding_86": -0.043308116, "title+abstract_embedding_87": -0.12620564, "title+abstract_embedding_88": -0.48540363, "title+abstract_embedding_89": -0.058725737, "title+abstract_embedding_90": 0.2874152, "title+abstract_embedding_91": 0.000357386, "title+abstract_embedding_92": -0.020940676, "title+abstract_embedding_93": 0.046238877, "title+abstract_embedding_94": 0.23496115, "title+abstract_embedding_95": -0.05557666, "title+abstract_embedding_96": 0.17773138, "title+abstract_embedding_97": -0.048753217, "title+abstract_embedding_98": 0.00118608, "title+abstract_embedding_99": 0.059528984, "title+abstract_embedding_100": 0.10941856, "title+abstract_embedding_101": -0.2387514, "title+abstract_embedding_102": 0.05520927, "title+abstract_embedding_103": 0.025813729, "title+abstract_embedding_104": 0.25327328, "title+abstract_embedding_105": 0.11376333, "title+abstract_embedding_106": -0.10868332, "title+abstract_embedding_107": 0.003245822, "title+abstract_embedding_108": -0.14849778, "title+abstract_embedding_109": 0.046790376, "title+abstract_embedding_110": 0.11244732, "title+abstract_embedding_111": 0.27393082, "title+abstract_embedding_112": 0.043182775, "title+abstract_embedding_113": -0.004550576, "title+abstract_embedding_114": 0.22322184, "title+abstract_embedding_115": 0.049019564, "title+abstract_embedding_116": 0.20102976, "title+abstract_embedding_117": -0.17756034, "title+abstract_embedding_118": -0.025598578, "title+abstract_embedding_119": 0.13760749, "title+abstract_embedding_120": -0.14624798, "title+abstract_embedding_121": -0.05881925, "title+abstract_embedding_122": -0.110716075, "title+abstract_embedding_123": 0.15136877, "title+abstract_embedding_124": 0.039812595, "title+abstract_embedding_125": 0.10351123, "title+abstract_embedding_126": -0.02117543, "title+abstract_embedding_127": 0.04311557, "label": 3, "label-multi": "19;3" }, { "paper_new_id": 71, "id": "j_5035aa321c38d7e59d6c17982feb308e", "title+abstract": "When Layered Nickela??Cobalt Silicate Hydroxide Nanosheets Meet Carbon Nanotubes: A Synergetic Coaxial Nanocable Structure for Enhanced Electrocatalytic Water Oxidation;Developing robust earth-abundant electrocatalysts for oxygen evolution reaction (OER) is an ongoing scientific challenge, which is coupled with a number of important electrochemical processes and many key renewable energy systems, such as water splitting, rechargeable metal-air batteries, and regenerative fuel cells. Here, we proposed a rational design and fabrication of the synergetic coaxial nanocable structures by intimate growth of the layered nickel-cobalt silicate hydroxide nanosheets on the outer surfaces of multiwalled carbon nanotubes (MWCNTs@NCS) and demonstrated their high efficiency in electrocatalytic OER from water splitting. The electrocatalytic activities of the MWCNTs@NCS were found to be significantly higher than that of bare NCS and pristine MWCNTs, synergetically determining by such the constituted individual components. Among them, the MWCNTs@NCS-2 exhibited best electrocatalytic OER performance, showing a small OER onset potential, large anodic current and long-term durability, which was favorably comparable to the previously reported NiCo-based OER electrocatalysts in alkaline electrolytes. To the best of our knowledge, this was a first example on the earth-abundant metal silicate hydroxides utilized in electrochemical water splitting.", "title+abstract_embedding_0": -0.27868462, "title+abstract_embedding_1": -1.0569711, "title+abstract_embedding_2": -0.9350275, "title+abstract_embedding_3": -0.4815904, "title+abstract_embedding_4": 0.3159426, "title+abstract_embedding_5": 0.10175729, "title+abstract_embedding_6": -0.42852893, "title+abstract_embedding_7": -0.4279018, "title+abstract_embedding_8": -0.4840465, "title+abstract_embedding_9": -0.10730052, "title+abstract_embedding_10": -0.34747225, "title+abstract_embedding_11": -0.13195637, "title+abstract_embedding_12": -0.13133422, "title+abstract_embedding_13": 0.21652192, "title+abstract_embedding_14": 0.766837, "title+abstract_embedding_15": -0.3309266, "title+abstract_embedding_16": 0.18685836, "title+abstract_embedding_17": 0.46636757, "title+abstract_embedding_18": -0.01454559, "title+abstract_embedding_19": 0.18991487, "title+abstract_embedding_20": -0.1478726, "title+abstract_embedding_21": 0.26001415, "title+abstract_embedding_22": -0.09140601, "title+abstract_embedding_23": -0.17414917, "title+abstract_embedding_24": 0.20203915, "title+abstract_embedding_25": -0.09045094, "title+abstract_embedding_26": -0.094441816, "title+abstract_embedding_27": -0.24371105, "title+abstract_embedding_28": -0.11404395, "title+abstract_embedding_29": 0.08987287, "title+abstract_embedding_30": -0.17359014, "title+abstract_embedding_31": -0.2555605, "title+abstract_embedding_32": 0.26058045, "title+abstract_embedding_33": -0.1847347, "title+abstract_embedding_34": -0.18769991, "title+abstract_embedding_35": 0.052433856, "title+abstract_embedding_36": -0.0691019, "title+abstract_embedding_37": 0.24836423, "title+abstract_embedding_38": -0.036061633, "title+abstract_embedding_39": 0.104804814, "title+abstract_embedding_40": -0.23420757, "title+abstract_embedding_41": -0.03203116, "title+abstract_embedding_42": 0.057063133, "title+abstract_embedding_43": -0.20169024, "title+abstract_embedding_44": 0.16973905, "title+abstract_embedding_45": 0.010009825, "title+abstract_embedding_46": -0.024504185, "title+abstract_embedding_47": 0.17129341, "title+abstract_embedding_48": -0.10414834, "title+abstract_embedding_49": -0.071394295, "title+abstract_embedding_50": -0.09680727, "title+abstract_embedding_51": -0.1751329, "title+abstract_embedding_52": -0.006248832, "title+abstract_embedding_53": -0.3938638, "title+abstract_embedding_54": 0.023770124, "title+abstract_embedding_55": 0.01502602, "title+abstract_embedding_56": -0.10993245, "title+abstract_embedding_57": -0.116561614, "title+abstract_embedding_58": -0.15923363, "title+abstract_embedding_59": -0.07980518, "title+abstract_embedding_60": -0.057588935, "title+abstract_embedding_61": -0.19955304, "title+abstract_embedding_62": -0.25416112, "title+abstract_embedding_63": -0.016587224, "title+abstract_embedding_64": 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"title+abstract_embedding_87": -0.07187757, "title+abstract_embedding_88": -0.034301177, "title+abstract_embedding_89": -0.04900939, "title+abstract_embedding_90": 0.09830297, "title+abstract_embedding_91": -0.001028009, "title+abstract_embedding_92": 0.10344197, "title+abstract_embedding_93": -0.009972952, "title+abstract_embedding_94": -0.12571122, "title+abstract_embedding_95": -0.06005335, "title+abstract_embedding_96": 0.008623399, "title+abstract_embedding_97": -0.15889382, "title+abstract_embedding_98": 0.049877614, "title+abstract_embedding_99": -0.08401038, "title+abstract_embedding_100": 0.008551396, "title+abstract_embedding_101": 0.033673003, "title+abstract_embedding_102": -0.19230154, "title+abstract_embedding_103": -0.09249609, "title+abstract_embedding_104": -0.1214225, "title+abstract_embedding_105": 0.11244372, "title+abstract_embedding_106": -0.010782301, "title+abstract_embedding_107": 0.11565366, "title+abstract_embedding_108": -0.07697102, "title+abstract_embedding_109": 0.026570752, "title+abstract_embedding_110": 0.20451325, "title+abstract_embedding_111": -0.22644389, "title+abstract_embedding_112": -0.03191279, "title+abstract_embedding_113": -0.13542093, "title+abstract_embedding_114": -0.024123892, "title+abstract_embedding_115": 0.041698385, "title+abstract_embedding_116": -0.00542479, "title+abstract_embedding_117": 0.026131105, "title+abstract_embedding_118": -0.076254465, "title+abstract_embedding_119": -0.050976697, "title+abstract_embedding_120": -0.19538555, "title+abstract_embedding_121": 0.11753797, "title+abstract_embedding_122": 0.016430289, "title+abstract_embedding_123": -0.03772285, "title+abstract_embedding_124": -0.034756966, "title+abstract_embedding_125": -0.04334896, "title+abstract_embedding_126": -0.040706836, "title+abstract_embedding_127": 0.002875611, "label": 1, "label-multi": "1;15" }, { "paper_new_id": 72, "id": "j_5129c318c8b76318b526d551d7161101", "title+abstract": "Tailoring carbon nanotubes surface with maleic anhydride for highly dispersed PtRu nanoparticles and their electrocatalytic oxidation of methanol;Based on carboxylated-carbon nanotubes (CNT-C) prepared by a direct Friedel¡§CCrafts reaction between pristine CNTs and maleic anhydride, PtRu nanoparticles are highly dispersed on the CNT-C surface and showed superb performance towards methanol electrooxidation.
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"title+abstract_embedding_113": 0.074488744, "title+abstract_embedding_114": 0.10365054, "title+abstract_embedding_115": 0.0839076, "title+abstract_embedding_116": 0.17983013, "title+abstract_embedding_117": 0.005425759, "title+abstract_embedding_118": 0.114980265, "title+abstract_embedding_119": 0.044962663, "title+abstract_embedding_120": -0.022174977, "title+abstract_embedding_121": 0.0964145, "title+abstract_embedding_122": 0.020049334, "title+abstract_embedding_123": -0.08856966, "title+abstract_embedding_124": 0.14594616, "title+abstract_embedding_125": 0.2084235, "title+abstract_embedding_126": 0.081738845, "title+abstract_embedding_127": -0.0978456, "label": 3, "label-multi": "3" }, { "paper_new_id": 73, "id": "j_51dd77563f4dc3acf87282eff44a6d92", "title+abstract": "Synergistic effects of surface Lewis Base/Acid and nitrogen defect in MgAl layered double Oxides/Carbon nitride heterojunction for efficient photoreduction of carbon dioxide;Abstract Conversion of CO2 to CO from solar energy on semiconductors is a promising route to renewable energy, but their practicality is limited by the poor adsorption and activation of CO2 on the semiconductor surface and the low utilization of photovoltaic carriers. Here, we construct a MgAl layered double oxide/nitrogen-deficient carbon nitride (MgAl LDO/Nv-CN) nanosheets hybrid by in situ deposition of MgAl layered double hydroxide (MgAl LDH) on Nv-CN nanosheets followed by subsequent calcination. The MgAl LDO serves as the surface-rich Lewis basic sites to effectively enhance adsorption of CO2 and H2O, while the nitrogen defects can enhance the optical absorption of g-C3N4 and improve the charge carrier separation. The optimal MgAl LDO/Nv-CN has high photocatalytic activity for CO2 reduction with a CO generation rate of 20.47 |¨¬mol?¡èg-1?¡èh-1 under visible light illumination, which is 6 times higher than that of bulk g-C3N4. Our work highlights the significance of synergy of MgAl LDO Lewis base/acid sites and nitrogen vacancy defects in the design of efficient photocatalysts for CO2 reduction.", "title+abstract_embedding_0": 0.5242976, "title+abstract_embedding_1": 0.3764398, "title+abstract_embedding_2": -0.2853569, "title+abstract_embedding_3": -0.7340437, "title+abstract_embedding_4": 0.25480455, "title+abstract_embedding_5": -0.25198895, "title+abstract_embedding_6": 0.004956126, "title+abstract_embedding_7": -0.49141893, "title+abstract_embedding_8": -0.10686156, "title+abstract_embedding_9": -0.22690588, "title+abstract_embedding_10": 0.067834884, "title+abstract_embedding_11": -0.45382994, "title+abstract_embedding_12": -0.1344162, "title+abstract_embedding_13": 0.5530435, "title+abstract_embedding_14": -0.17479353, "title+abstract_embedding_15": 0.055433314, "title+abstract_embedding_16": -0.19827035, "title+abstract_embedding_17": -0.18120977, "title+abstract_embedding_18": -0.04490807, 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Surfactant-Thermal Method to Prepare Two Novel Two-Dimensional Mn-Sb-S Compounds for Photocatalytic Applications.;The new two-dimensional compounds (IV) and (VII) crystallize in the monoclinic space group C2/c with Z = 4 (single crystal XRD).", "title+abstract_embedding_0": -1.0492941, "title+abstract_embedding_1": 0.77858007, "title+abstract_embedding_2": -0.21012571, "title+abstract_embedding_3": -0.007260323, "title+abstract_embedding_4": -0.6231226, "title+abstract_embedding_5": 0.37750643, "title+abstract_embedding_6": 0.1490117, "title+abstract_embedding_7": 1.0321826, "title+abstract_embedding_8": 0.24072818, "title+abstract_embedding_9": 0.58652663, "title+abstract_embedding_10": -0.14265785, "title+abstract_embedding_11": -0.551422, "title+abstract_embedding_12": -0.3917865, "title+abstract_embedding_13": -0.34848186, "title+abstract_embedding_14": -0.09256981, "title+abstract_embedding_15": -0.17209029, "title+abstract_embedding_16": 0.13264868, "title+abstract_embedding_17": 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"j_53020fa4b6915277cba1372d5cdbbc45", "title+abstract": "Unraveling the Lighta??Activated Reaction Mechanism in a Catalytically Competent Key Intermediate of a Multifunctional Molecular Catalyst for Artificial Photosynthesis;Abstract Understanding photodriven multielectron reaction pathways requires the identification and spectroscopic characterization of intermediates and their excited?\\state dynamics, which is very challenging due to their short lifetimes. To the best of our knowledge, this manuscript reports for the first time on in?situ spectroelectrochemistry as an alternative approach to study the excited?\\state properties of reactive intermediates of photocatalytic cycles. UV/Vis, resonance?\\Raman, and transient?\\absorption spectroscopy have been employed to characterize the catalytically competent intermediate (tbbpy)2RuII(tpphz)RhICp*] of [(tbbpy)2Ru(tpphz)Rh(Cp*)Cl]Cl(PF6)2 (Ru(tpphz)RhCp*), a photocatalyst for the hydrogenation of nicotinamide (NAD?\\analogue) and proton reduction, generated by electrochemical and chemical reduction. Electronic transitions shifting electron density from the activated catalytic center to the bridging tpphz ligand significantly reduce the catalytic activity upon visible?\\light irradiation.", "title+abstract_embedding_0": 0.14679027, "title+abstract_embedding_1": 0.6059491, "title+abstract_embedding_2": 1.0183997, "title+abstract_embedding_3": -1.314887, "title+abstract_embedding_4": -0.10892612, "title+abstract_embedding_5": 0.25475925, "title+abstract_embedding_6": 0.20600781, "title+abstract_embedding_7": 0.31755129, "title+abstract_embedding_8": 0.16245306, "title+abstract_embedding_9": -0.18947113, "title+abstract_embedding_10": 0.58702636, "title+abstract_embedding_11": -0.28107923, "title+abstract_embedding_12": 0.2859798, "title+abstract_embedding_13": -0.28967196, "title+abstract_embedding_14": -0.2539464, "title+abstract_embedding_15": 0.27202195, "title+abstract_embedding_16": 0.13896382, "title+abstract_embedding_17": 0.3900064, "title+abstract_embedding_18": 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"title+abstract_embedding_108": 0.055355012, "title+abstract_embedding_109": 0.075254574, "title+abstract_embedding_110": 0.24762857, "title+abstract_embedding_111": 0.002884947, "title+abstract_embedding_112": -0.016737819, "title+abstract_embedding_113": -0.012760088, "title+abstract_embedding_114": 0.014164299, "title+abstract_embedding_115": 0.087381475, "title+abstract_embedding_116": -0.13128403, "title+abstract_embedding_117": 0.023267344, "title+abstract_embedding_118": 0.06062068, "title+abstract_embedding_119": -0.20583515, "title+abstract_embedding_120": -0.016518923, "title+abstract_embedding_121": -0.04988744, "title+abstract_embedding_122": 0.061353147, "title+abstract_embedding_123": -0.03497393, "title+abstract_embedding_124": 0.10506299, "title+abstract_embedding_125": -0.040381975, "title+abstract_embedding_126": -0.014979949, "title+abstract_embedding_127": -0.058490828, "label": 3, "label-multi": "3" }, { "paper_new_id": 76, "id": "j_530b610e6699ce610b5dc3602eb02593", "title+abstract": "Insights into Compositional and Structural Effects of Bimetallic Hollow Mesoporous Nanospheres toward Ethanol Oxidation Electrocatalysis;A one-pot soft-templating method is reported to fabricate nanosized bimetallic PdAg hollow mesoporous nanospheres (HMSs) for electrocatalytic ethanol oxidation reaction (EOR). The synthesis relies on the \"dual-template\" surfactant of dioctadecyldimethylammonium chloride that drives in-situ growth of mesoporous frameworks on the surface of vesicles into the HMSs with radially opened mesochannels. The synthetic protocol is extendable to engineer elemental compositions and hierarchical nanostructures of PdAg nanoalloys. This system thus provides a direct yet solid platform to understand catalytic add-in synergies toward electrochemical EOR. By evaluating compositional and structural features separately, bimetallic Pd65Ag35 HMSs display the highest EOR activity with a mass activity of 4.61 A mgPd-1. Mechanism studies indicate synergistically electronic and bifunctional effects as well as structural advantages of Pd65Ag35 HMSs kinetically optimize the removal of poisoning carbonaceous intermediates and accelerate the diffusion processes (the rate-determining step), thus promoting the EOR performance accordingly.", "title+abstract_embedding_0": -0.19002676, "title+abstract_embedding_1": -0.9105101, "title+abstract_embedding_2": -0.14504543, "title+abstract_embedding_3": -0.21332157, "title+abstract_embedding_4": -0.053981245, "title+abstract_embedding_5": 0.953689, "title+abstract_embedding_6": -0.39665177, "title+abstract_embedding_7": 0.04548584, "title+abstract_embedding_8": -0.44666716, "title+abstract_embedding_9": 0.482945, "title+abstract_embedding_10": 0.018335417, "title+abstract_embedding_11": 0.16170576, "title+abstract_embedding_12": -0.02405572, "title+abstract_embedding_13": 0.38911262, "title+abstract_embedding_14": 0.3853623, "title+abstract_embedding_15": 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"label-multi": "1;15;2;3" }, { "paper_new_id": 77, "id": "j_5465af967a06eb8567c18546215eacdd", "title+abstract": "Photocatalytic activity of ZnO doped with Ag on the degradation of endocrine disrupting under UV irradiation and the investigation of its antibacterial activity;Abstract Ag-doped ZnO photocatalysts with different Ag molar content (0.0, 0.5, 1.0, 2.0 and 4.0%) were prepared via hydrothermal method. The X-ray diffraction (XRD), Nitrogen physisorption at 77?K, Fourier transformed infrared spectroscopy (FTIR), UV¡§C-Visible spectroscopy, Photoluminescence spectra (PL) and Raman spectroscopy were used to characterize the structural, textural and optical properties of the samples. The results showed that Ag-doping does not change the average crystallite size with the Ag low content (?¨¹1.0%) but slightly decreases with Ag high content (>1.0%). The specific surface area (SBET) increases with the increase of the Ag content. The band gap values of ZnO are decreased with the increase of the Ag doping level. The results of the photocatalytic degradation of bisphenol A (BPA) and nonylphenol (NP) in aqueous solutions under UV irradiation and in the presence of hydrogen peroxide (H2O2) showed that silver ions doping greatly improved the photocatalytic efficiency of ZnO. The TOC conversion BPA and NP are 72.1% and 81.08% respectively obtained using 1% Ag-doped ZnO. The enhancement of photocatalytic activity is ascribed to the fact that the modification of ZnO with an appropriate amount of Ag can increase the separation efficiency of the photogenerated electrons-holes in ZnO. The antibacterial activity of the catalysts which uses Escherichia coli as a model for Gram-negative bacteria confirmed that Ag-doped ZnO possessed more antibacterial activity than the pure ZnO.", "title+abstract_embedding_0": 1.1354815, "title+abstract_embedding_1": 0.37843305, "title+abstract_embedding_2": 0.21419281, "title+abstract_embedding_3": -0.12197065, "title+abstract_embedding_4": -0.24745709, "title+abstract_embedding_5": -1.1604125, "title+abstract_embedding_6": 0.1722088, "title+abstract_embedding_7": 0.16512832, "title+abstract_embedding_8": 0.17403863, "title+abstract_embedding_9": 0.3783089, "title+abstract_embedding_10": -0.21556512, "title+abstract_embedding_11": 0.35546112, "title+abstract_embedding_12": 0.4796428, "title+abstract_embedding_13": -0.058374144, "title+abstract_embedding_14": -0.21104693, "title+abstract_embedding_15": 0.32397825, "title+abstract_embedding_16": -0.08257404, "title+abstract_embedding_17": -0.08386706, "title+abstract_embedding_18": 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"j_5612c4e5938553c3a88fa66a73cc6f79", "title+abstract": "Electrocatalytic hydrogen evolution by cobalt difluoroboryl-diglyoximate complexes;In the presence of moderately strong acids in CH3CN, cobalt complexes with BF2-bridged diglyoxime ligands are active catalysts for the reduction of protons to H2 at potentials as positive as -0.28 V vs. SCE.", "title+abstract_embedding_0": -2.4694464, "title+abstract_embedding_1": -0.16388664, "title+abstract_embedding_2": 0.2563952, "title+abstract_embedding_3": -0.84946954, "title+abstract_embedding_4": 0.5984703, "title+abstract_embedding_5": 0.055401325, "title+abstract_embedding_6": 0.0767543, "title+abstract_embedding_7": 0.17313996, "title+abstract_embedding_8": 0.06961159, "title+abstract_embedding_9": -0.20316428, "title+abstract_embedding_10": 0.12082417, "title+abstract_embedding_11": 0.22322741, "title+abstract_embedding_12": 0.24010442, "title+abstract_embedding_13": -0.73390156, "title+abstract_embedding_14": 0.17218706, 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"label-multi": "3" }, { "paper_new_id": 79, "id": "j_566e359c7316e367c07f68559588ab27", "title+abstract": "Thiosulfate enhanced degradation of organic pollutants in aqueous solution with g-C3N4 under visible light irradiation;Developing new strategies to design more practicable and efficient g-C3N4 based photocatalysts is important to solve the environmental issues. Thiosulfate (STS) is a common residual product found in wastewater and removal of STS remains a matter of great environmental concern. In this work, however, STS is activated by g-C3N4 under visible light irradiation, resulting in a fast degradation of Rhodamine B (RhB) and other pollutants. The performance of g-C3N4 prepared from urea was much higher than that from melamine, due to the higher surface area and more negative conduction band potential of the former catalyst. In addition, comparison with other oxidants and reductants such as peroxymonosulfate, peroxydisulfate, hydrogen peroxide and sulfite, the use of STS in g-C3N4/Vis system showed the highest efficiency for RhB degradation. During ten successive cycles, the excellent reusability of the catalyst was also obtained. The effect of different concentrations of STS and g-C3N4, and initial solution pH on the performance of the system were also studied. The mechanism study suggests that STS is first oxidized to S2O3- radicals by photohole, which will be transformed to other oxysulfur radicals such as SO3- and finally to SO42- ions. At the same time, the rate of O2 reduction by photoelectrons to O2- radicals as well as RhB degradation increases. The finding of this study provides a promising advanced oxidation process for organic pollutants degradation via STS activation.", "title+abstract_embedding_0": 0.5171602, "title+abstract_embedding_1": 0.20859408, "title+abstract_embedding_2": 1.3337994, "title+abstract_embedding_3": -0.30785453, "title+abstract_embedding_4": -0.3508879, "title+abstract_embedding_5": 0.060857058, "title+abstract_embedding_6": -0.35013804, "title+abstract_embedding_7": -0.31933126, "title+abstract_embedding_8": 0.5567926, "title+abstract_embedding_9": 0.13860252, "title+abstract_embedding_10": 0.0931714, "title+abstract_embedding_11": 0.40775803, "title+abstract_embedding_12": 0.18168978, "title+abstract_embedding_13": 0.28868, "title+abstract_embedding_14": -0.15588874, "title+abstract_embedding_15": -0.03509278, "title+abstract_embedding_16": -0.13957572, "title+abstract_embedding_17": -0.37011847, "title+abstract_embedding_18": 0.115101665, "title+abstract_embedding_19": -0.10998608, 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"title+abstract_embedding_110": 0.07461023, "title+abstract_embedding_111": 0.18011665, "title+abstract_embedding_112": -0.020037696, "title+abstract_embedding_113": 0.05860375, "title+abstract_embedding_114": 0.014430121, "title+abstract_embedding_115": -0.014700733, "title+abstract_embedding_116": -0.022004694, "title+abstract_embedding_117": -0.022668883, "title+abstract_embedding_118": -0.15785693, "title+abstract_embedding_119": 0.12582432, "title+abstract_embedding_120": -0.07923273, "title+abstract_embedding_121": -0.06621384, "title+abstract_embedding_122": -0.078694075, "title+abstract_embedding_123": -0.13202721, "title+abstract_embedding_124": 0.25709692, "title+abstract_embedding_125": 0.09966002, "title+abstract_embedding_126": -0.15018144, "title+abstract_embedding_127": -0.05305384, "label": 16, "label-multi": "16" }, { "paper_new_id": 80, "id": "j_56f479578f74c47d2fd60611c01423f3", "title+abstract": "The effect of extended conjugation on electrocatalytic CO2 reduction by molecular catalysts and macromolecular structures;Abstract Homogenous molecular catalysts have shown significant promise for the selective reduction of CO2 to single products. However, their practical application in emerging CO2 reduction technologies is hindered by their limited solubility and stability in aqueous solutions, their diffusion-dependent kinetics, and their poor recyclability. Incorporating discrete molecular catalysts into macromolecular architectures such as covalent organic frameworks is one solution to these limitations that allows for the synthesis of heterogeneous materials with increased activity and stability but that still maintain the selectivity and active-site tunability of discrete molecular catalysts. Forming such macromolecular materials necessarily extends the ligand |D-conjugated network, which can have important effects on the electrocatalytic activity. In this review, we discuss recent studies on the effect of extended |D-conjugation on the catalytic activity of molecular catalyst and extended macromolecular architectures, with an emphasis on how activity is influenced by charge delocalization, electrostatic effects, and electronic coupling between active sites.", "title+abstract_embedding_0": -0.58948016, "title+abstract_embedding_1": -0.6516878, "title+abstract_embedding_2": 0.1534836, "title+abstract_embedding_3": -0.62711, "title+abstract_embedding_4": 0.0859012, "title+abstract_embedding_5": 0.94689655, "title+abstract_embedding_6": -0.5304152, "title+abstract_embedding_7": 0.18927887, "title+abstract_embedding_8": 0.20204702, "title+abstract_embedding_9": 0.25464252, "title+abstract_embedding_10": 0.10611433, "title+abstract_embedding_11": -0.23180552, "title+abstract_embedding_12": 0.43298703, "title+abstract_embedding_13": 0.056304462, "title+abstract_embedding_14": 0.043581754, "title+abstract_embedding_15": -0.13907802, "title+abstract_embedding_16": 0.03565821, "title+abstract_embedding_17": -0.50529456, "title+abstract_embedding_18": 0.0981819, "title+abstract_embedding_19": -0.01071135, "title+abstract_embedding_20": 0.5162533, "title+abstract_embedding_21": 0.20937741, "title+abstract_embedding_22": 0.19903214, "title+abstract_embedding_23": 0.2968651, "title+abstract_embedding_24": -0.009028763, "title+abstract_embedding_25": 0.03645575, "title+abstract_embedding_26": -0.112821564, "title+abstract_embedding_27": 0.15970646, "title+abstract_embedding_28": -0.12943965, "title+abstract_embedding_29": 0.15164784, "title+abstract_embedding_30": 0.3051289, "title+abstract_embedding_31": 0.30587885, "title+abstract_embedding_32": -0.099797286, "title+abstract_embedding_33": 0.46022373, "title+abstract_embedding_34": 0.17619573, "title+abstract_embedding_35": 0.2897073, "title+abstract_embedding_36": 0.2831266, "title+abstract_embedding_37": -0.12173823, "title+abstract_embedding_38": 0.05649239, 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0.1319355, "title+abstract_embedding_107": -0.039645523, "title+abstract_embedding_108": -0.12474847, "title+abstract_embedding_109": 0.110751346, "title+abstract_embedding_110": 0.045298964, "title+abstract_embedding_111": -0.13766038, "title+abstract_embedding_112": -0.1343021, "title+abstract_embedding_113": 0.053186893, "title+abstract_embedding_114": 0.029318646, "title+abstract_embedding_115": -0.15813473, "title+abstract_embedding_116": -0.03738571, "title+abstract_embedding_117": 0.023472741, "title+abstract_embedding_118": -0.00711399, "title+abstract_embedding_119": -0.009567766, "title+abstract_embedding_120": 0.0777919, "title+abstract_embedding_121": 0.113193974, "title+abstract_embedding_122": 0.01514858, "title+abstract_embedding_123": 0.057337858, "title+abstract_embedding_124": 0.031690046, "title+abstract_embedding_125": 0.08317014, "title+abstract_embedding_126": 0.03704965, "title+abstract_embedding_127": 0.07735816, "label": 3, "label-multi": "1;14;3" }, { "paper_new_id": 81, "id": "j_58fca33b5410c21a422b63bf2ad2aeb3", "title+abstract": "One-pot synthesis of ultrafine NiO loaded and Ti3+ in-situ doped TiO2 induced by cyclodextrin for efficient visible-light photodegradation of hydrophobic pollutants;Inability to absorb visible light and fast recombination of photogenerated electrons and holes in TiO2 catalysts prevent their wide applications in photocatalysis. Herein, we report a novel strategy to in-situ synthesize Ti3+- doped TiO2 coupling with homo-dispersed NiO and beta-cyclodextrin (CD-Ni/TiO2). By using nickel stearate as precursor, ethyl acetoacetate and CD as chelating agents, porous CD-Ni/TiO2 nanospheres constructed by CD, ultrafine NiO (similar to 2 nm), and Ti3+-doped TiO2 (similar to 5 nm) are produced. The porous nanosphere structure enhances the surface utilization and electron-hole separation through intimate contact of NiO and TiO2. The doped Ti3+ extends the photo-response of TiO2 to visible region; while the CD structure with hydrophobic cavity endows CDNi/TiO2 with outstanding capability to entrap hydrophobic molecules. The CD-Ni/TiO2 with decreased band gap (2.70 eV) presents high activity and stability in visible-light photodegradation of hydrophobic pollutants. This study presents a simple strategy in TiO2 doping and activity enhancement through designing inorganic-organic composite photocatalyst for hydrophobic pollutant degradation under visible light.", "title+abstract_embedding_0": 0.83365166, "title+abstract_embedding_1": 0.71681094, "title+abstract_embedding_2": -0.9438044, "title+abstract_embedding_3": -0.1522367, "title+abstract_embedding_4": 0.4462455, "title+abstract_embedding_5": 0.2054056, "title+abstract_embedding_6": -0.57977057, "title+abstract_embedding_7": 0.2831536, "title+abstract_embedding_8": -0.52947736, "title+abstract_embedding_9": -0.07566929, "title+abstract_embedding_10": 0.14151752, "title+abstract_embedding_11": -0.25014028, "title+abstract_embedding_12": 0.19803953, "title+abstract_embedding_13": 0.21712524, "title+abstract_embedding_14": -0.10436548, "title+abstract_embedding_15": 0.03974484, "title+abstract_embedding_16": -0.21239838, "title+abstract_embedding_17": -0.24938002, "title+abstract_embedding_18": 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"title+abstract_embedding_64": 0.045752183, "title+abstract_embedding_65": -0.11377409, "title+abstract_embedding_66": -0.11551015, "title+abstract_embedding_67": -0.2087135, "title+abstract_embedding_68": -0.13092493, "title+abstract_embedding_69": 0.24957031, "title+abstract_embedding_70": -0.030066304, "title+abstract_embedding_71": -0.117202796, "title+abstract_embedding_72": 0.25765377, "title+abstract_embedding_73": 0.11635642, "title+abstract_embedding_74": -0.14727731, "title+abstract_embedding_75": -0.01365786, "title+abstract_embedding_76": 0.13757156, "title+abstract_embedding_77": 0.1335271, "title+abstract_embedding_78": 0.038250282, "title+abstract_embedding_79": 0.15246938, "title+abstract_embedding_80": 0.011934686, "title+abstract_embedding_81": 0.18233788, "title+abstract_embedding_82": -0.15621528, "title+abstract_embedding_83": -0.03490317, "title+abstract_embedding_84": 0.007348314, "title+abstract_embedding_85": 0.16209322, "title+abstract_embedding_86": 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"title+abstract_embedding_109": -0.052406594, "title+abstract_embedding_110": -0.06758511, "title+abstract_embedding_111": -0.04669599, "title+abstract_embedding_112": -0.12873586, "title+abstract_embedding_113": -0.110027924, "title+abstract_embedding_114": -0.012798056, "title+abstract_embedding_115": 0.06736277, "title+abstract_embedding_116": -0.034430355, "title+abstract_embedding_117": 0.010061596, "title+abstract_embedding_118": 0.004649446, "title+abstract_embedding_119": 0.009830304, "title+abstract_embedding_120": 0.061956864, "title+abstract_embedding_121": -0.074552834, "title+abstract_embedding_122": 0.064031616, "title+abstract_embedding_123": -0.057633333, "title+abstract_embedding_124": -0.13532051, "title+abstract_embedding_125": -0.063879095, "title+abstract_embedding_126": 0.06078379, "title+abstract_embedding_127": -0.05894798, "label": 0, "label-multi": "0" }, { "paper_new_id": 82, "id": "j_5afb7321a5a1d6ab157ebb93b1e68c9b", "title+abstract": "Fabrication of Bi-BiOCl/MgIn2S4 heterostructure with step-scheme mechanism for carbon dioxide photoreduction into methane;Abstract Step-scheme (S-scheme) Bi-BiOCl/MgIn2S4 heterostructure (BBOC/MIS) was successfully fabricated via NaBH4 reduction and facile in-situ hydrothermal process and applied in photocatalytic CO2 reduction. A part of BBOC ultrathin nanosheets processed by ultrasonication exfoliation was grown on the surfaces of MIS marigold microflower. Another part of BBOC and MIS exhibited as the core and shell of BBOC/MIS, respectively. The morphology, band alignment, optical and electronic characteristics of photocatalysts were comprehensively studied via diverse characterization methods. The S-scheme BBOC/MIS heterojunction possessed superior photocatalytic performance and well reusability to primarily convert CO2 into CH4 with high efficiency under the simulated solar light irradiation without using any sacrificial agent in water. Experimental results displayed that the 6% BBOC/MIS sample behaved the optimal photocatalytic performance in photocatalytic reduction of CO2, and its maximum CH4 production rate could reach up to 4.29 |¨¬mol g?1 h?1, which was about 7.56 times as high as that of unadulterated MIS. The enhanced photocatalytic performance of BBOC/MIS could be attributed to the improved visible light response and highly-efficient separation of the photogenerated electron-hole pairs between BBOC and MIS through the S-scheme heterojunction interface. In addition, the metal Bi acted as the bridge connecting the BOC and MIS to facilitate the charge transfer, which greatly promoted the CO2 photocatalytic reduction to CH4.", "title+abstract_embedding_0": 0.95832694, "title+abstract_embedding_1": 0.53566706, "title+abstract_embedding_2": 0.22084855, "title+abstract_embedding_3": -0.78607154, "title+abstract_embedding_4": -0.17299366, "title+abstract_embedding_5": 0.044327974, "title+abstract_embedding_6": -0.09529889, "title+abstract_embedding_7": -0.28266168, "title+abstract_embedding_8": -0.25656033, "title+abstract_embedding_9": -0.09264892, "title+abstract_embedding_10": 0.07980785, "title+abstract_embedding_11": 0.37605828, "title+abstract_embedding_12": -0.44668087, "title+abstract_embedding_13": -0.13624302, "title+abstract_embedding_14": -0.26401305, "title+abstract_embedding_15": 0.24269433, "title+abstract_embedding_16": 0.18624246, "title+abstract_embedding_17": -0.000990316, "title+abstract_embedding_18": -0.079217255, 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"title+abstract_embedding_109": -0.03326209, "title+abstract_embedding_110": -0.030602127, "title+abstract_embedding_111": -0.16778544, "title+abstract_embedding_112": -0.013427183, "title+abstract_embedding_113": 0.12673314, "title+abstract_embedding_114": -0.041624606, "title+abstract_embedding_115": 0.06295826, "title+abstract_embedding_116": -0.13785693, "title+abstract_embedding_117": -0.09274243, "title+abstract_embedding_118": -0.065433756, "title+abstract_embedding_119": -0.036684915, "title+abstract_embedding_120": 0.06747329, "title+abstract_embedding_121": 0.116295286, "title+abstract_embedding_122": 0.061463684, "title+abstract_embedding_123": 0.046344154, "title+abstract_embedding_124": -0.15111783, "title+abstract_embedding_125": -0.002038442, "title+abstract_embedding_126": 0.02580304, "title+abstract_embedding_127": 0.12915213, "label": 106, "label-multi": NaN }, { "paper_new_id": 83, "id": "j_5b81d8dae2310724e75ee4267270c654", "title+abstract": "Origin of Bulklike Structure and Bond Length Disorder of Pt37 and Pt6Ru31 Clusters on Carbon:a?? Comparison of Theory and Experiment;We describe a theoretical analysis of the structures of self-organizing nanoparticles formed by Pt and Ru-Pt on carbon support. The calculations provide insights into the nature of these metal particle systems-ones of current interest for use as the electrocatalytic materials of direct oxidation fuel cells-and clarify complex behaviors noted in earlier experimental studies. With clusters deposited via metallo-organic Pt or PtRu(5) complexes, previous experiments Nashner et al. J. Am. Chem. Soc. 1997, 119, 7760; Nashner et al. J. Am. Chem. Soc. 1998, 120, 8093; Frenkel et al. J. Phys. Chem. B 2001, 105, 12689] showed that the Pt and Pt-Ru based clusters are formed with fcc(111)-stacked cuboctahedral geometry and essentially bulklike metal-metal bond lengths, even for the smallest (few atom) nanoparticles for which the average coordination number is much smaller than that in the bulk, and that Pt in bimetallic [PtRu(5)] clusters segregates to the ambient surface of the supported nanoparticles. We explain these observations and characterize the cluster structures and bond length distributions using density functional theory calculations with graphite as a model for the support. The present study reveals the origin of the observed metal-metal bond length disorder, distinctively different for each system, and demonstrates the profound consequences that result from the cluster/carbon-support interactions and their key role in the structure and electronic properties of supported metallic nanoparticles.", "title+abstract_embedding_0": 0.42867422, "title+abstract_embedding_1": -0.92630833, "title+abstract_embedding_2": -0.14003208, "title+abstract_embedding_3": -0.30178165, "title+abstract_embedding_4": -0.27562267, "title+abstract_embedding_5": 1.119108, "title+abstract_embedding_6": 0.6699796, "title+abstract_embedding_7": 0.63184106, "title+abstract_embedding_8": 0.2910114, "title+abstract_embedding_9": -0.37202156, "title+abstract_embedding_10": -0.20646998, "title+abstract_embedding_11": -0.35397348, "title+abstract_embedding_12": 0.14614165, "title+abstract_embedding_13": -0.3889225, "title+abstract_embedding_14": 0.20006293, "title+abstract_embedding_15": 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"label": 3, "label-multi": "3" }, { "paper_new_id": 84, "id": "j_5cde1a085eb54d602189ac9a64493f5c", "title+abstract": "Remarkable charge separation and photocatalytic efficiency enhancement through TiO2(B)/anatase hetrophase junctions of TiO2 nanobelts;Abstract Light harvesting and charge separation are both significant to the photocatalysis, but it is challenging to synchronously realize both in a single-component material. The surface coarsened TiO2 nanobelts with TiO2(B)/anatase hetrophase junctions and large BET surface area are prepared via a hydrothermal/annealing method. The presence of surface coarsened nanobelt structure enhances the light absorption through reflection/refraction of light. The TiO2(B)/anatase hetrophase junctions can efficiently promote the separation of photoinduced electrons and holes pairs and therefore decrease the charge recombination. The large BET surface area provides abundant active sites for the absorption and diffusion of reactants. As a consequence, the obtained TiO2 nanobelts exhibit an enhanced photocatalytic H2 evolution activity at the optimal annealing temperature (450???C) with Pt as co-catalysts (0.786?mmol?h?1g?1), exceeding that of pure anatase TiO2 nanobelts (TiO2 nanobelts-600???C, 0.265?mmol?h?1g?1). Interestingly, TiO2 nanobelts-450???C still show a high hydrogen evolution rate of 0.601?mmol?h?1g?1 in the absence of co-catalysts.", "title+abstract_embedding_0": 0.7548727, "title+abstract_embedding_1": 0.5395563, "title+abstract_embedding_2": -0.67850065, "title+abstract_embedding_3": -0.2803073, "title+abstract_embedding_4": 0.5505981, "title+abstract_embedding_5": 0.43681186, "title+abstract_embedding_6": 0.402802, "title+abstract_embedding_7": -0.15951486, "title+abstract_embedding_8": -0.6022892, "title+abstract_embedding_9": -0.19930685, "title+abstract_embedding_10": -0.25608802, "title+abstract_embedding_11": -0.418408, "title+abstract_embedding_12": -0.03783703, "title+abstract_embedding_13": 0.1290574, "title+abstract_embedding_14": -0.27953827, "title+abstract_embedding_15": -0.27533445, "title+abstract_embedding_16": 0.04680255, "title+abstract_embedding_17": 0.0835039, "title+abstract_embedding_18": 0.2168846, "title+abstract_embedding_19": 0.13392593, 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"title+abstract_embedding_110": 0.12387702, "title+abstract_embedding_111": 0.11514542, "title+abstract_embedding_112": 0.03285472, "title+abstract_embedding_113": -0.08659871, "title+abstract_embedding_114": 0.1489177, "title+abstract_embedding_115": -0.019630529, "title+abstract_embedding_116": 0.11346446, "title+abstract_embedding_117": -0.121711016, "title+abstract_embedding_118": -0.04713318, "title+abstract_embedding_119": 0.01873135, "title+abstract_embedding_120": 0.011762921, "title+abstract_embedding_121": 0.16189803, "title+abstract_embedding_122": -0.18912515, "title+abstract_embedding_123": -0.08422994, "title+abstract_embedding_124": 0.07140473, "title+abstract_embedding_125": 0.07054474, "title+abstract_embedding_126": 0.007324539, "title+abstract_embedding_127": -0.053771093, "label": 106, "label-multi": NaN }, { "paper_new_id": 85, "id": "j_5d827a41aa77d81bfa8d5dc77db6e8bf", "title+abstract": "Template-Directed Assembly of Metala??Chalcogenide Nanocrystals into Ordered Mesoporous Networks;Although great progress in the synthesis of porous networks of metal and metal oxide nanoparticles with highly accessible pore surface and ordered mesoscale pores has been achieved, synthesis of assembled 3D mesostructures of metal-chalcogenide nanocrystals is still challenging. In this work we demonstrate that ordered mesoporous networks, which comprise well-defined interconnected metal sulfide nanocrystals, can be prepared through a polymer-templated oxidative polymerization process. The resulting self-assembled mesostructures that were obtained after solvent extraction of the polymer template impart the unique combination of light-emitting metal chalcogenide nanocrystals, three-dimensional open-pore structure, high surface area, and uniform pores. We show that the pore surface of these materials is active and accessible to incoming molecules, exhibiting high photocatalytic activity and stability, for instance, in oxidation of 1-phenylethanol into acetophenone. We demonstrate through appropriate selection of the synthetic components that this method is general to prepare ordered mesoporous materials from metal chalcogenide nanocrystals with various sizes and compositions.", "title+abstract_embedding_0": 0.10341859, "title+abstract_embedding_1": -0.59112686, "title+abstract_embedding_2": -0.84514904, "title+abstract_embedding_3": -0.36279786, "title+abstract_embedding_4": -0.61106277, "title+abstract_embedding_5": 1.0293465, "title+abstract_embedding_6": -0.4485326, "title+abstract_embedding_7": 0.3598762, "title+abstract_embedding_8": -0.20745629, "title+abstract_embedding_9": 0.26062912, "title+abstract_embedding_10": -0.086729646, "title+abstract_embedding_11": -0.2862567, "title+abstract_embedding_12": -0.089660466, "title+abstract_embedding_13": 0.42138973, "title+abstract_embedding_14": 0.5433848, "title+abstract_embedding_15": -0.25286657, "title+abstract_embedding_16": 0.22922117, "title+abstract_embedding_17": -0.11284116, 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a??artificial catalysta?? in situ formed from CdTe QDs and inorganic cobalt salts for photocatalytic hydrogen evolution;A simple hollow-structured \"artificial catalyst\" in situ formed from CdTe QDs and CoCl2 center dot 6H(2)O in aqueous ascorbic acid solution has shown exceptional activity and stability for photocatalytic H-2 evolution (25 mu mol h(-1) mg(-1), 219 100 mol H-2 per mol QDs or 59 600 mol H-2 per mol Co turnovers, respectively) under visible light irradiation for 70 h.", "title+abstract_embedding_0": -0.5936325, "title+abstract_embedding_1": 0.7988043, "title+abstract_embedding_2": 0.46769905, "title+abstract_embedding_3": -0.746117, "title+abstract_embedding_4": 0.50605375, "title+abstract_embedding_5": 0.19136685, "title+abstract_embedding_6": 0.47653946, "title+abstract_embedding_7": -0.07288414, "title+abstract_embedding_8": 0.6262695, "title+abstract_embedding_9": -0.1122933, "title+abstract_embedding_10": -0.117258266, "title+abstract_embedding_11": 0.10983604, 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"title+abstract_embedding_125": 0.19210951, "title+abstract_embedding_126": 0.002874926, "title+abstract_embedding_127": 0.0477753, "label": 3, "label-multi": "0;16;17;3" }, { "paper_new_id": 87, "id": "j_5f9f99e7d3686836e54ce1c64bf436b0", "title+abstract": "Fine-tuning internal electric field of BiOBr for suppressed charge recombination;Abstract Owing to the potential to solve environmental issues, semiconductor photocatalysis process using solar energy has drawn significant attention in recent decades. So, the photocatalysis major issues have solved by semiconductor nanotechnology. Here, BiOBr layered structures are synthesized with induced IEF, oxygen vacancies, and layer growth along 001} direction by using hydrothermal synthesis method. Therefore, we exercise optimized amounts of EG, which organized Bi ions at the surface of BiOBr. The exposed {001} facet orientation and oxygen vacancy generation are controlled by using EG. Consequently, the bonding force of the Bi-O band is reduced, allowing O atoms to be dragged out under solar light irradiation, resulting oxygen vacancies produced. Finally, these oxygen vacancies induced IEF across the layers of BiOBr, which suppressed electrons-holes recombination and enhanced reaction process with the degraded material achieved. Most significantly, optimized EG quantity has used to the synthesis of BiOBr structures, which improve photogenerated electrons holes (e?-h+) pairs capability due to IEF and oxygen vacancies. Thus, an optimized quantity of EG is a strategic measure to induce IEF, which is significant for separation of (e?-h+) pairs, consequently, it enhances photocatalytic performance and has considered a novel method.", "title+abstract_embedding_0": -0.055511832, "title+abstract_embedding_1": -0.4668473, "title+abstract_embedding_2": 0.51140976, "title+abstract_embedding_3": -0.30535543, "title+abstract_embedding_4": -0.7078582, "title+abstract_embedding_5": -0.13848978, "title+abstract_embedding_6": 0.44829625, "title+abstract_embedding_7": -0.5735575, "title+abstract_embedding_8": -0.32510188, "title+abstract_embedding_9": -0.02374643, "title+abstract_embedding_10": 0.05899717, "title+abstract_embedding_11": 0.3223132, "title+abstract_embedding_12": 0.005775124, "title+abstract_embedding_13": 0.08498711, "title+abstract_embedding_14": -0.23248377, "title+abstract_embedding_15": 0.53656125, "title+abstract_embedding_16": -0.07655741, "title+abstract_embedding_17": 0.061890304, 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"title+abstract_embedding_108": 0.11182493, "title+abstract_embedding_109": 0.12267192, "title+abstract_embedding_110": -0.1729353, "title+abstract_embedding_111": 0.08995845, "title+abstract_embedding_112": -0.004535034, "title+abstract_embedding_113": 0.039704643, "title+abstract_embedding_114": 0.12822446, "title+abstract_embedding_115": -0.001190901, "title+abstract_embedding_116": -0.16406024, "title+abstract_embedding_117": -0.012194529, "title+abstract_embedding_118": 0.10664052, "title+abstract_embedding_119": -0.09847729, "title+abstract_embedding_120": 0.32829064, "title+abstract_embedding_121": -0.10807268, "title+abstract_embedding_122": -0.0902234, "title+abstract_embedding_123": -0.11306657, "title+abstract_embedding_124": 0.22260125, "title+abstract_embedding_125": -0.10725031, "title+abstract_embedding_126": 0.033196792, "title+abstract_embedding_127": -0.110526145, "label": 106, "label-multi": NaN }, { "paper_new_id": 88, "id": "j_62db0442c4c60f36564549f2fabe9926", "title+abstract": "A new steric tetra-imidazole for facile synthesis of high loading atomically dispersed FeN4 electrocatalysts;Abstract Atomically dispersed FeN4 rich carbon-based electrocatalysts obtained by pyrolysis of Zn-based metal-organic frameworks (mainly Fe modified ZIF-8) exhibits remarkable catalytic performance for oxygen reduction reaction (ORR). However, the independence of each ZIF-8 particle with rhomb dodecahedral results in a physical stack and undesirable charge transfer path and subsequently induce the iron buried in the carbon matrix after the pyrolysis process, which further impedes the high loading of atomic iron (usually less than 1?wt%). Herein, we newly designed a novel steric tetra-imidazole structure to anchor iron in a cross way. This strategy achieves the synthesis of atomically dispersed FeN4 rich carbon-based electrocatalyst in one-step approach without any pretreatment and/or further acid leaching. Unlike the traditional imidazole in ZIF-8, the novel steric tetra-imidazole structure exhibits a benzene ring located in the center of each four imidazole groups acting as sharing side-chain substitution, which can control the distance of each metal rivet center and impede the aggregation of iron effectively. The obtained catalyst, named as TimB-Fe5-C, exhibits high atomic iron loading content up to 2.58?wt% and exhibits efficient ORR electrocatalytic performance in both alkaline and acid medium. Significantly, this new steric tetra-imidazole endows one-step facile synthesis of atomically dispersed electrocatalysts with high loading and to avoid unpredictable changes of structure brought by tedious pre-treatment as well as post-treatment.", "title+abstract_embedding_0": 0.15116858, "title+abstract_embedding_1": -0.9678798, "title+abstract_embedding_2": -0.3359861, "title+abstract_embedding_3": -1.0480664, "title+abstract_embedding_4": 0.32464844, "title+abstract_embedding_5": -0.10616869, "title+abstract_embedding_6": -0.34026042, "title+abstract_embedding_7": 0.26159325, "title+abstract_embedding_8": -0.12873183, "title+abstract_embedding_9": 0.5312327, "title+abstract_embedding_10": -0.16419576, "title+abstract_embedding_11": 0.0977273, "title+abstract_embedding_12": 0.54138684, "title+abstract_embedding_13": -0.20031986, "title+abstract_embedding_14": -0.084319994, "title+abstract_embedding_15": -0.26263988, "title+abstract_embedding_16": -0.38170248, 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"j_63590e0f54e6711fb5982357cec6991a", "title+abstract": "Supramolecular Packing Controls H2 Photocatalysis in Chromophore Amphiphile Hydrogels;Light harvesting supramolecular assemblies are potentially useful structures as components of solar-to-fuel conversion materials. The development of these functional constructs requires an understanding of optimal packing modes for chromophores. We investigated here assembly in water and the photocatalytic function of perylene monoimide chromophore amphiphiles with different alkyl linker lengths separating their hydrophobic core and the hydrophilic carboxylate headgroup. We found that these chromophore amphiphiles (CAs) self-assemble into charged nanostructures of increasing aspect ratio as the linker length is increased. The addition of salt to screen the charged nanostructures induced the formation of hydrogels and led to internal crystallization within some of the nanostructures. For linker lengths up to seven methylenes, the CAs were found to pack into 2D crystalline unit cells within ribbon-shaped nanostructures, whereas the nine methylene CAs assembled into long nanofibers without crystalline molecular packing. At the same time, the different molecular packing arrangements after charge screening led to different absorbance spectra, despite the identical electronic properties of all PMI amphiphiles. While the crystalline CAs formed electronically coupled H-aggregates, only CAs with intermediate linker lengths showed evidence of high intermolecular orbital overlap. Photocatalytic hydrogen production using a nickel-based catalyst was observed in all hydrogels, with the highest turnovers observed for CA gels having intermediate linker lengths. We conclude that the improved photocatalytic performance of the hydrogels formed by supramolecular assemblies of the intermediate linker CA molecules likely arises from improved exciton splitting efficiencies due to their higher orbital overlap.", "title+abstract_embedding_0": 0.8337382, "title+abstract_embedding_1": -0.13443053, "title+abstract_embedding_2": -0.00255841, "title+abstract_embedding_3": -0.7166208, "title+abstract_embedding_4": -0.52084816, "title+abstract_embedding_5": 0.60014886, "title+abstract_embedding_6": -0.23217878, "title+abstract_embedding_7": -0.2104877, "title+abstract_embedding_8": -0.34538585, "title+abstract_embedding_9": -0.3375138, "title+abstract_embedding_10": -0.025995567, "title+abstract_embedding_11": -0.07396154, "title+abstract_embedding_12": -0.178363, "title+abstract_embedding_13": -0.2461645, "title+abstract_embedding_14": 0.16192469, "title+abstract_embedding_15": -0.07158373, "title+abstract_embedding_16": -0.11388445, 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"title+abstract_embedding_108": -0.09975899, "title+abstract_embedding_109": 0.006876379, "title+abstract_embedding_110": 0.026159883, "title+abstract_embedding_111": 0.155669, "title+abstract_embedding_112": -0.07375048, "title+abstract_embedding_113": 0.11411377, "title+abstract_embedding_114": 0.038918436, "title+abstract_embedding_115": 0.008804232, "title+abstract_embedding_116": 0.01051943, "title+abstract_embedding_117": 0.14468727, "title+abstract_embedding_118": 0.04016453, "title+abstract_embedding_119": 0.10038477, "title+abstract_embedding_120": 0.028618708, "title+abstract_embedding_121": 0.10955218, "title+abstract_embedding_122": 0.037759706, "title+abstract_embedding_123": -0.019622378, "title+abstract_embedding_124": 0.053569373, "title+abstract_embedding_125": 0.007090509, "title+abstract_embedding_126": 0.13078554, "title+abstract_embedding_127": 0.110136986, "label": 3, "label-multi": "3" }, { "paper_new_id": 90, "id": "j_690e62717131dfa34ee7cb9133a2d511", "title+abstract": "Fabrication of Z-scheme Bi3O4Cl/g-C3N4 2D/2D heterojunctions with enhanced interfacial charge separation and photocatalytic degradation various organic pollutants activity;A novel Z-scheme Bi3O4Cl/g-C3N4 2D/2D heterojunctions were successfully prepared by solid phase calcination method. The Z-scheme Bi3O4Cl/g-C3N4 2D/2D heterojunctions exhibit outstanding photocatalytic activity for removing the various water contaminant under visible light, such as antibiotic, dye and heavy metal. The enhancement of phototcatalytic performance is ascribed to the interfacial interaction between 2D Bi3O4Cl nanoflakes and 2D g-C3N4 nanosheets, which can enlarge specific surface area and improve separation efficiency of photogenerated electron-hole pairs. To explain the interfacial interaction between Bi3O4Cl and g-C-3 N-4 in Z-scheme Bi3O4Cl/g-C3N4 2D/2D heterojunctions, the transmission electron microscopy, X-ray photoelectron spectroscopy and N-2 adsorption-desorption isotherms measurements were investigated. In addition, the photocatalytic mechanism over Z-scheme Bi3O4Cl/g-C3N4 2D/2D heterojunction is systematically investigated by the calculation, trapping experimental and ESR technology. The present work may provide a promising approach to fabrication of other Z-scheme 2D/2D heterojunction with efficient photocatalytic activity.", "title+abstract_embedding_0": 0.95605624, "title+abstract_embedding_1": 0.51752186, "title+abstract_embedding_2": -0.38687095, "title+abstract_embedding_3": -0.7663375, "title+abstract_embedding_4": -0.2935483, "title+abstract_embedding_5": -0.35033995, "title+abstract_embedding_6": -0.27741143, "title+abstract_embedding_7": 0.33744568, "title+abstract_embedding_8": -0.3135294, "title+abstract_embedding_9": 0.15621606, "title+abstract_embedding_10": -0.09853358, "title+abstract_embedding_11": 0.13431577, "title+abstract_embedding_12": 0.06999265, "title+abstract_embedding_13": -0.001749521, "title+abstract_embedding_14": -0.0945939, "title+abstract_embedding_15": -0.10602248, "title+abstract_embedding_16": -0.045674518, "title+abstract_embedding_17": -0.1982387, "title+abstract_embedding_18": 0.18171169, "title+abstract_embedding_19": 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"title+abstract_embedding_110": 0.018219799, "title+abstract_embedding_111": 0.06722381, "title+abstract_embedding_112": -0.059748396, "title+abstract_embedding_113": -0.004753128, "title+abstract_embedding_114": 0.113868654, "title+abstract_embedding_115": 0.084102064, "title+abstract_embedding_116": 0.054336816, "title+abstract_embedding_117": 0.04374343, "title+abstract_embedding_118": 0.11635636, "title+abstract_embedding_119": -0.1708574, "title+abstract_embedding_120": -0.10276513, "title+abstract_embedding_121": -0.014358627, "title+abstract_embedding_122": -0.12308073, "title+abstract_embedding_123": 0.11959692, "title+abstract_embedding_124": -0.012043439, "title+abstract_embedding_125": 0.22026223, "title+abstract_embedding_126": -0.0109572, "title+abstract_embedding_127": 0.050765835, "label": 3, "label-multi": "1;2;3" }, { "paper_new_id": 91, "id": "j_6adf94806671eba24541f050ab70f3f3", "title+abstract": "Electronic structurea??sunlight driven water splitting activity correlation of (Zn1a??yGay)(O1a??zNz);(Zn1-yGay)(O1-zNz) (y?¨¹ 0.10; z?¨¹ 0.15) solid solutions have been investigated for their electronic structure and visible light photocatalytic activity, and a correlation was found between them. (Zn1-yGay)(O1-zNz) with ZnO as the major component have been synthesized by a solution combustion method in 10 minutes using simple raw materials. The local structures of Zn K edge and Ga K edge, and changes in the chemical environment with the incorporation of Ga and N in ZnO were determined by EXAFS study. EXAFS and XRD results suggested the dissolution of GaN in the ZnO lattice. The homogeneity of the solid solution was demonstrated from HRTEM studies. Photoluminescence studies revealed the creation of a new band at the top of the ZnO valence band (VB), and thus the broadening of the VB of (Zn1-yGay)(O1-zNz) or a decrease in the band gap was attributed to the origin of visible light absorption. UV-Vis spectral studies showed light absorption up to 550 nm, which directly supports the VB broadening. Predominant oxygen vacancies and high photocorrosion observed for ZnO were fully suppressed for (Zn1-yGay)(O1-zNz), indicating the minimization of defects, and thus more sustainability under irradiation conditions. The bare solid solution exhibited reasonable and promising activity for solar hydrogen evolution and photoelectrochemical current generation at 0 V. The present work explained factors such as the preparation method, single phase structure with the stabilization of integral parts, homogeneity in the structure, compensation of oxygen vacancies, and suppression of the density of recombination centres that play a pivotal role in realizing solar energy harvesting.", "title+abstract_embedding_0": 0.8472339, "title+abstract_embedding_1": -0.2180366, "title+abstract_embedding_2": 0.3156188, "title+abstract_embedding_3": -0.25963974, "title+abstract_embedding_4": -0.46243834, "title+abstract_embedding_5": -1.0448108, "title+abstract_embedding_6": 0.6841999, "title+abstract_embedding_7": 0.24025087, "title+abstract_embedding_8": 0.07319314, "title+abstract_embedding_9": 0.17205739, "title+abstract_embedding_10": -0.20940606, "title+abstract_embedding_11": -0.4809326, "title+abstract_embedding_12": 0.46371046, "title+abstract_embedding_13": 0.14368415, "title+abstract_embedding_14": -0.016636312, "title+abstract_embedding_15": 0.254448, 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"label-multi": "2;3" }, { "paper_new_id": 92, "id": "j_6d61b8e435441ce02bc5ab680b287766", "title+abstract": "The effect of gold on platinum oxidation in homogeneous Aua??Pt electrocatalysts;Abstract Oxidation of Au¡§CPt thin films was carried out in ambient air at room temperature and characterized by X-ray photoelectron spectroscopy. The homogeneous films were prepared by RF co-sputtering with concentrations varying from Au 9 Pt 91 to Au 89 Pt 11 and compared to pure Pt and Au thin films. Spectral deconvolution of the Au 4 f and Pt 4 f core levels revealed linear peak shifts for both the Au¡§CAu and Pt¡§CPt bonding components as a function of alloy mixture and metallic component peak asymmetry that remained constant for all alloy stoichiometries. The predominant oxidation products were PtO and PtO 2 and were characterized by stable core level binding energies for all films. A gradual decline in the Pt¡§CO x products and corresponding levels of elemental oxygen was observed with increasing Au content but was similar in proportion to the metallic Pt components. Based on these results, variations in Pt oxide phases and/or concentration do not appear to contribute to enhanced electrocatalytic activity for oxygen reduction observed for the intermediate alloy stoichiometries.", "title+abstract_embedding_0": 0.15949976, "title+abstract_embedding_1": -0.60113543, "title+abstract_embedding_2": 0.24020572, "title+abstract_embedding_3": 0.31305516, "title+abstract_embedding_4": 0.52049667, "title+abstract_embedding_5": 0.04776615, "title+abstract_embedding_6": 1.3335686, "title+abstract_embedding_7": 0.3035825, "title+abstract_embedding_8": 0.965299, "title+abstract_embedding_9": -0.9102093, "title+abstract_embedding_10": 0.08578691, "title+abstract_embedding_11": 0.7269065, "title+abstract_embedding_12": 0.3480842, "title+abstract_embedding_13": 0.21932024, "title+abstract_embedding_14": 0.029361933, "title+abstract_embedding_15": -0.12715821, "title+abstract_embedding_16": -0.46396536, "title+abstract_embedding_17": 0.18339634, "title+abstract_embedding_18": 0.41341418, "title+abstract_embedding_19": 0.22674356, "title+abstract_embedding_20": -0.05916223, "title+abstract_embedding_21": -0.0735114, "title+abstract_embedding_22": 0.40294883, "title+abstract_embedding_23": -0.07943395, "title+abstract_embedding_24": 0.10893446, "title+abstract_embedding_25": 0.22347355, "title+abstract_embedding_26": 0.10868165, "title+abstract_embedding_27": 0.1514822, "title+abstract_embedding_28": 0.12436212, "title+abstract_embedding_29": -0.5260303, "title+abstract_embedding_30": -0.030755773, "title+abstract_embedding_31": -0.2701207, "title+abstract_embedding_32": 0.01799994, "title+abstract_embedding_33": 0.01086548, "title+abstract_embedding_34": -0.06897712, "title+abstract_embedding_35": 0.03904789, "title+abstract_embedding_36": -0.32061985, "title+abstract_embedding_37": 0.045337185, "title+abstract_embedding_38": 0.07319684, "title+abstract_embedding_39": -0.37246475, "title+abstract_embedding_40": 0.006436497, "title+abstract_embedding_41": -0.19264635, "title+abstract_embedding_42": 0.1494444, "title+abstract_embedding_43": 0.16793631, "title+abstract_embedding_44": -0.3765477, "title+abstract_embedding_45": -0.012704641, "title+abstract_embedding_46": 0.3971906, "title+abstract_embedding_47": 0.20955482, "title+abstract_embedding_48": 0.055261835, "title+abstract_embedding_49": 0.112486646, "title+abstract_embedding_50": 0.001846567, "title+abstract_embedding_51": 0.07365833, "title+abstract_embedding_52": -0.005965099, "title+abstract_embedding_53": -0.02490934, "title+abstract_embedding_54": 0.07828005, "title+abstract_embedding_55": 0.006980714, "title+abstract_embedding_56": 0.13049923, "title+abstract_embedding_57": -0.04177095, "title+abstract_embedding_58": 0.32304436, "title+abstract_embedding_59": 0.062200278, "title+abstract_embedding_60": -0.18800893, "title+abstract_embedding_61": 0.05317985, "title+abstract_embedding_62": 0.049952812, "title+abstract_embedding_63": -0.3540528, "title+abstract_embedding_64": 0.27168214, "title+abstract_embedding_65": -0.058148373, "title+abstract_embedding_66": 0.05089962, "title+abstract_embedding_67": -0.05991167, "title+abstract_embedding_68": -0.053422563, "title+abstract_embedding_69": 0.3798231, "title+abstract_embedding_70": -0.20530316, "title+abstract_embedding_71": 0.10486017, "title+abstract_embedding_72": -0.31922594, "title+abstract_embedding_73": 0.034699254, "title+abstract_embedding_74": -0.04491853, "title+abstract_embedding_75": 0.111381814, "title+abstract_embedding_76": -0.09151298, "title+abstract_embedding_77": -0.1603777, "title+abstract_embedding_78": 0.018576235, "title+abstract_embedding_79": -0.018871874, "title+abstract_embedding_80": -0.033087846, "title+abstract_embedding_81": 0.009208977, "title+abstract_embedding_82": 0.19978075, "title+abstract_embedding_83": 0.11183028, "title+abstract_embedding_84": 0.022919491, "title+abstract_embedding_85": -0.06970494, "title+abstract_embedding_86": 0.09472266, "title+abstract_embedding_87": 0.0940263, "title+abstract_embedding_88": -0.05061818, "title+abstract_embedding_89": 0.1037166, "title+abstract_embedding_90": -0.09194144, "title+abstract_embedding_91": 0.053796776, "title+abstract_embedding_92": -0.15688986, "title+abstract_embedding_93": 0.19354138, "title+abstract_embedding_94": 0.007101923, "title+abstract_embedding_95": -0.11328161, "title+abstract_embedding_96": 0.10581062, "title+abstract_embedding_97": -0.034904484, "title+abstract_embedding_98": 0.09208998, "title+abstract_embedding_99": 0.056881674, "title+abstract_embedding_100": 0.010357909, "title+abstract_embedding_101": -0.06717778, "title+abstract_embedding_102": 0.057890892, "title+abstract_embedding_103": -0.2702562, "title+abstract_embedding_104": 0.086149685, "title+abstract_embedding_105": -0.046098456, "title+abstract_embedding_106": -0.028296113, "title+abstract_embedding_107": -0.007850071, "title+abstract_embedding_108": 0.057419837, "title+abstract_embedding_109": 0.08849953, "title+abstract_embedding_110": 0.04195562, "title+abstract_embedding_111": -0.17595437, "title+abstract_embedding_112": -0.10500096, "title+abstract_embedding_113": 0.08392015, "title+abstract_embedding_114": 0.062067166, "title+abstract_embedding_115": -0.40430704, "title+abstract_embedding_116": 0.061027836, "title+abstract_embedding_117": -0.13460267, "title+abstract_embedding_118": 0.032406162, "title+abstract_embedding_119": 0.009899739, "title+abstract_embedding_120": 0.033043567, "title+abstract_embedding_121": 0.021644538, "title+abstract_embedding_122": -0.06284276, "title+abstract_embedding_123": -0.012755021, "title+abstract_embedding_124": 0.10152893, "title+abstract_embedding_125": 0.20786706, "title+abstract_embedding_126": 0.07319162, "title+abstract_embedding_127": -0.07911654, "label": 3, "label-multi": "1;2;3" }, { "paper_new_id": 93, "id": "j_6d7f6a458982df0e64ef27ce54d8c928", "title+abstract": "Correlation between microstructure and property of electroless deposited Pt counter electrodes on plastic substrate for dye-sensitized solar cells;Flexible Pt counter electrodes (CEs) were prepared on indium-doped tin oxide coated polyethylene naphthalate (ITO-PEN) substrate by electroless deposition. The correlation between the microstructure and the property of the Pt CEs was investigated. Results showed that isolated Pt nanoparticles were uniformly distributed on the ITO surface at a short deposition duration, and then grew with the deposition duration, leading to the interconnection of adjacent Pt nanoparticles. The interconnection of Pt nanoparticles was beneficial to the electrical property of the Pt CEs, while it was unfavorable to the electrocatalytic property of the Pt CEs. A microstructure model was proposed to explain the correlation between the microstructure and the property of the Pt CEs. In addition, the Pt CEs showed low charge transfer resistance (1.66-0.58 Omega cm(2)), which was comparable to that (1.16 Omega cm(2)) of the conventional sputtered Pt CE. The high electrocatalytic property of the electroless deposited Pt CEs makes the assembled DSCs present comparable energy conversion efficiency of the DSCs using sputtered Pt CE. (C) 2011 Elsevier B.V. All rights reserved.", "title+abstract_embedding_0": -0.03877306, "title+abstract_embedding_1": -0.7694051, "title+abstract_embedding_2": -0.5627918, "title+abstract_embedding_3": 0.8825245, "title+abstract_embedding_4": -0.42280874, "title+abstract_embedding_5": 0.25487104, "title+abstract_embedding_6": 0.8315842, "title+abstract_embedding_7": -0.22213066, "title+abstract_embedding_8": 0.20359354, "title+abstract_embedding_9": -0.86305475, "title+abstract_embedding_10": -0.18879882, "title+abstract_embedding_11": -0.09442029, "title+abstract_embedding_12": 0.27022237, "title+abstract_embedding_13": -0.095458224, "title+abstract_embedding_14": -0.44955269, "title+abstract_embedding_15": 0.25794575, "title+abstract_embedding_16": 0.22846138, "title+abstract_embedding_17": -0.4327099, "title+abstract_embedding_18": 0.062761456, "title+abstract_embedding_19": -0.17990968, "title+abstract_embedding_20": 0.14516784, "title+abstract_embedding_21": -0.31326908, "title+abstract_embedding_22": 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"title+abstract_embedding_68": 0.33913594, "title+abstract_embedding_69": 0.17910239, "title+abstract_embedding_70": 0.31969738, "title+abstract_embedding_71": 0.21444531, "title+abstract_embedding_72": -0.029341705, "title+abstract_embedding_73": -0.11780313, "title+abstract_embedding_74": 0.04528924, "title+abstract_embedding_75": -0.20645419, "title+abstract_embedding_76": 0.0177418, "title+abstract_embedding_77": -0.14623134, "title+abstract_embedding_78": 0.10902849, "title+abstract_embedding_79": 0.014621973, "title+abstract_embedding_80": -0.14592044, "title+abstract_embedding_81": -0.15665847, "title+abstract_embedding_82": -0.10966763, "title+abstract_embedding_83": -0.016902635, "title+abstract_embedding_84": 0.12322981, "title+abstract_embedding_85": -0.00625387, "title+abstract_embedding_86": -0.14365709, "title+abstract_embedding_87": 0.033048812, "title+abstract_embedding_88": -0.14032249, "title+abstract_embedding_89": -0.07415227, "title+abstract_embedding_90": 0.04174407, "title+abstract_embedding_91": -0.15363476, "title+abstract_embedding_92": -0.12705696, "title+abstract_embedding_93": -0.008001111, "title+abstract_embedding_94": 0.17815426, "title+abstract_embedding_95": 0.04696004, "title+abstract_embedding_96": 0.09657254, "title+abstract_embedding_97": 0.13314886, "title+abstract_embedding_98": 0.15409435, "title+abstract_embedding_99": -0.035157047, "title+abstract_embedding_100": -0.18547946, "title+abstract_embedding_101": 0.007242411, "title+abstract_embedding_102": -0.012333982, "title+abstract_embedding_103": -0.106520206, "title+abstract_embedding_104": 0.040240213, "title+abstract_embedding_105": 0.07525173, "title+abstract_embedding_106": -0.1070303, "title+abstract_embedding_107": 0.070167005, "title+abstract_embedding_108": -0.14598048, "title+abstract_embedding_109": 0.010948092, "title+abstract_embedding_110": 0.15743011, "title+abstract_embedding_111": 0.2000381, "title+abstract_embedding_112": -0.014152482, "title+abstract_embedding_113": -0.049988165, "title+abstract_embedding_114": 0.0388114, "title+abstract_embedding_115": 0.008899123, "title+abstract_embedding_116": 0.060981855, "title+abstract_embedding_117": -0.105658665, "title+abstract_embedding_118": 0.17560507, "title+abstract_embedding_119": 0.21822433, "title+abstract_embedding_120": -0.24841158, "title+abstract_embedding_121": -0.05925911, "title+abstract_embedding_122": -0.028679132, "title+abstract_embedding_123": 0.09645989, "title+abstract_embedding_124": 0.08275314, "title+abstract_embedding_125": -0.035025828, "title+abstract_embedding_126": -0.10618391, "title+abstract_embedding_127": 0.123485185, "label": 3, "label-multi": "1;2;3" }, { "paper_new_id": 94, "id": "j_6ea3fde1fd255c4bd2a76cb479d9c53e", "title+abstract": "Direct Observation of Reactive Trapped Holes in TiO2 Undergoing Photocatalytic Oxidation of Adsorbed Alcohols:a?? Evaluation of the Reaction Rates and Yields;To investigate the primary process of photocatalytic oxidation of TiO2, interfacial charge-transfer reaction of trapped holes formed in nanocrystalline TiO2 films by UV irradiation was directly measured by highly sensitive femtosecond and nanosecond transient absorption spectroscopy under low intensity excitation condition to avoid fast electron-hole recombination. Accordingly, the rates and yields of photocatalytic oxidation of several alcohols adsorbed on TiO2 were evaluated successfully.", "title+abstract_embedding_0": -0.35628277, "title+abstract_embedding_1": 1.4264048, "title+abstract_embedding_2": -0.1512753, "title+abstract_embedding_3": 0.9452702, "title+abstract_embedding_4": 1.0195236, "title+abstract_embedding_5": 0.29310188, "title+abstract_embedding_6": 0.18648715, "title+abstract_embedding_7": 0.019147344, "title+abstract_embedding_8": -0.39113462, "title+abstract_embedding_9": -0.18366587, "title+abstract_embedding_10": 0.57771987, "title+abstract_embedding_11": -0.03067051, "title+abstract_embedding_12": 0.16672081, "title+abstract_embedding_13": -0.14333662, "title+abstract_embedding_14": 0.05122724, "title+abstract_embedding_15": -0.4896382, "title+abstract_embedding_16": 0.46580303, "title+abstract_embedding_17": -0.33552694, "title+abstract_embedding_18": 0.2712949, "title+abstract_embedding_19": -0.0998594, "title+abstract_embedding_20": -0.29567128, "title+abstract_embedding_21": 0.03865446, "title+abstract_embedding_22": 0.1530499, "title+abstract_embedding_23": -0.22250064, "title+abstract_embedding_24": -0.0341969, "title+abstract_embedding_25": 0.16592264, "title+abstract_embedding_26": -0.47380766, "title+abstract_embedding_27": 0.027578318, "title+abstract_embedding_28": -0.054418385, "title+abstract_embedding_29": 0.31442234, "title+abstract_embedding_30": 0.063397616, "title+abstract_embedding_31": -0.030286152, "title+abstract_embedding_32": 0.17429271, "title+abstract_embedding_33": 0.33173698, "title+abstract_embedding_34": 0.19126926, "title+abstract_embedding_35": -0.22182998, "title+abstract_embedding_36": -0.18539073, "title+abstract_embedding_37": 0.3222866, "title+abstract_embedding_38": 0.007380098, "title+abstract_embedding_39": 0.031973712, "title+abstract_embedding_40": -0.22483099, "title+abstract_embedding_41": 0.11264123, "title+abstract_embedding_42": -0.27160275, "title+abstract_embedding_43": -0.28010768, "title+abstract_embedding_44": -0.1260447, "title+abstract_embedding_45": 0.03553477, "title+abstract_embedding_46": 0.4441073, "title+abstract_embedding_47": -0.03951514, "title+abstract_embedding_48": 0.07171154, "title+abstract_embedding_49": -0.1457488, "title+abstract_embedding_50": 0.2158526, "title+abstract_embedding_51": -0.17533925, "title+abstract_embedding_52": 0.056013614, "title+abstract_embedding_53": 0.14370163, "title+abstract_embedding_54": 0.02817826, "title+abstract_embedding_55": 0.05092124, "title+abstract_embedding_56": -0.07716082, "title+abstract_embedding_57": 0.1893146, "title+abstract_embedding_58": 0.14009215, "title+abstract_embedding_59": -0.05080624, "title+abstract_embedding_60": -0.0924167, "title+abstract_embedding_61": -0.095101915, "title+abstract_embedding_62": 0.082507074, "title+abstract_embedding_63": -0.022083499, "title+abstract_embedding_64": -0.21899109, "title+abstract_embedding_65": -0.077623434, "title+abstract_embedding_66": -0.10604524, "title+abstract_embedding_67": 0.035348, "title+abstract_embedding_68": 0.17483027, "title+abstract_embedding_69": -0.15063092, "title+abstract_embedding_70": -0.09511622, "title+abstract_embedding_71": -0.22926944, "title+abstract_embedding_72": -0.34856212, "title+abstract_embedding_73": -0.00115157, "title+abstract_embedding_74": -0.19579929, "title+abstract_embedding_75": 0.083606586, "title+abstract_embedding_76": 0.063142836, "title+abstract_embedding_77": -0.43686533, "title+abstract_embedding_78": 0.08318612, "title+abstract_embedding_79": 0.23597425, "title+abstract_embedding_80": 0.08094417, "title+abstract_embedding_81": 0.34021133, "title+abstract_embedding_82": -0.27479738, "title+abstract_embedding_83": -0.068161614, "title+abstract_embedding_84": 0.035594672, "title+abstract_embedding_85": -0.15931319, "title+abstract_embedding_86": -0.05102142, "title+abstract_embedding_87": -0.024456766, "title+abstract_embedding_88": 0.06691784, "title+abstract_embedding_89": -0.1417706, "title+abstract_embedding_90": -0.09464646, "title+abstract_embedding_91": -4.42e-05, "title+abstract_embedding_92": -0.043696843, "title+abstract_embedding_93": 0.2052722, "title+abstract_embedding_94": -0.09246796, "title+abstract_embedding_95": -0.048078947, "title+abstract_embedding_96": -0.07942591, "title+abstract_embedding_97": -0.17508869, "title+abstract_embedding_98": -0.16780525, "title+abstract_embedding_99": 0.12263908, "title+abstract_embedding_100": 0.09485093, "title+abstract_embedding_101": 0.29492164, "title+abstract_embedding_102": -0.03835641, "title+abstract_embedding_103": 0.04440151, "title+abstract_embedding_104": -0.25614092, "title+abstract_embedding_105": -0.03214878, "title+abstract_embedding_106": -0.13731194, "title+abstract_embedding_107": -0.19680803, "title+abstract_embedding_108": 0.03801824, "title+abstract_embedding_109": 0.006182671, "title+abstract_embedding_110": 0.04380551, "title+abstract_embedding_111": 0.030294217, "title+abstract_embedding_112": -0.094963476, "title+abstract_embedding_113": -0.08762273, "title+abstract_embedding_114": -0.114607885, "title+abstract_embedding_115": -0.001227781, "title+abstract_embedding_116": -0.16852452, "title+abstract_embedding_117": -0.14846958, "title+abstract_embedding_118": 0.10899785, "title+abstract_embedding_119": -0.046647206, "title+abstract_embedding_120": 0.046376366, "title+abstract_embedding_121": 0.11344059, "title+abstract_embedding_122": 0.11246392, "title+abstract_embedding_123": 0.17465979, "title+abstract_embedding_124": -0.09822724, "title+abstract_embedding_125": -0.15753666, "title+abstract_embedding_126": 0.027718037, "title+abstract_embedding_127": -0.07669407, "label": 3, "label-multi": "3" }, { "paper_new_id": 95, "id": "j_70ce4a12330e88bb71fa887f40ee325c", "title+abstract": "Adsorption and photocatalytic degradation of acetonitrile: FT-IR investigation;Abstract The photocatalytic degradation of acetonitrile was carried out in liquid¡§Csolid regime in a batch reactor by using two types of commercial TiO 2 powders (Merck and Degussa P25) as photocatalysts. The concentration of acetonitrile and non-purgeable organic carbon (NPOC) were monitored. The initial rate of acetonitrile conversion was found higher on TiO 2 Merck than on TiO 2 P25. FT-IR spectroscopy was used to investigate the molecular features of the adsorption and photo-oxidation of acetonitrile on the two TiO 2 powders in a fully surface hydrated form. Acetonitrile was found adsorbed on Ti 4+ surface ions and hydroxyl groups for both types of TiO 2 . This interaction appeared fully reversible in the case of the Merck photocatalyst, whereas acetonitrile was more strongly stabilized on Ti 4+ ions of TiO 2 P25. Furthermore, the adsorption of CD 3 CN?Ti 4+ on this type of photocatalyst resulted in the formation of acetamide-like species, because of the presence of nucleophilic surface O 2? and hydroxyl groups. The formation of these species, strongly bound to the TiO 2 surface and recalcitrant to the photo-oxidation, could result in the poisoning of a part of the photocatalytic sites of TiO 2 P25, accounting for its lower initial acetonitrile conversion rate.", "title+abstract_embedding_0": 0.97673786, "title+abstract_embedding_1": 0.8834709, "title+abstract_embedding_2": 0.49588293, "title+abstract_embedding_3": 0.37977278, "title+abstract_embedding_4": 0.6420621, "title+abstract_embedding_5": 0.16886595, "title+abstract_embedding_6": -0.29381868, "title+abstract_embedding_7": 0.26071995, "title+abstract_embedding_8": -0.3299485, "title+abstract_embedding_9": -0.43623555, "title+abstract_embedding_10": 0.3869214, "title+abstract_embedding_11": -0.0240038, "title+abstract_embedding_12": -0.010095179, "title+abstract_embedding_13": 0.003835347, "title+abstract_embedding_14": 0.007864893, "title+abstract_embedding_15": -0.40996638, "title+abstract_embedding_16": 0.024465859, "title+abstract_embedding_17": -0.001702845, "title+abstract_embedding_18": 0.22022258, "title+abstract_embedding_19": 0.067601584, "title+abstract_embedding_20": 0.30664057, "title+abstract_embedding_21": -0.4731759, "title+abstract_embedding_22": 0.14032361, "title+abstract_embedding_23": -0.10702616, "title+abstract_embedding_24": -0.053906664, "title+abstract_embedding_25": 0.024828196, "title+abstract_embedding_26": 0.002627477, "title+abstract_embedding_27": -0.32094347, "title+abstract_embedding_28": 0.14110142, "title+abstract_embedding_29": -0.22910778, "title+abstract_embedding_30": -0.11762646, "title+abstract_embedding_31": -0.013203437, "title+abstract_embedding_32": 0.09109859, "title+abstract_embedding_33": -0.028043315, "title+abstract_embedding_34": -0.112225264, "title+abstract_embedding_35": 0.007863931, "title+abstract_embedding_36": 0.1905435, "title+abstract_embedding_37": 0.17569207, "title+abstract_embedding_38": -0.043930933, "title+abstract_embedding_39": 0.20237312, "title+abstract_embedding_40": 0.17216483, "title+abstract_embedding_41": 0.088288955, "title+abstract_embedding_42": 0.060283303, "title+abstract_embedding_43": -0.059116334, "title+abstract_embedding_44": -0.17554665, "title+abstract_embedding_45": 0.08962953, "title+abstract_embedding_46": 0.006603152, "title+abstract_embedding_47": -0.087938726, "title+abstract_embedding_48": -0.19387998, "title+abstract_embedding_49": 0.21330321, "title+abstract_embedding_50": 0.24366184, "title+abstract_embedding_51": -0.2982341, "title+abstract_embedding_52": 0.062439904, "title+abstract_embedding_53": -0.12745707, "title+abstract_embedding_54": 0.114796236, "title+abstract_embedding_55": -0.001002457, "title+abstract_embedding_56": -0.09727462, "title+abstract_embedding_57": -0.12409424, "title+abstract_embedding_58": -0.052690163, "title+abstract_embedding_59": 0.03166713, "title+abstract_embedding_60": -0.09597811, "title+abstract_embedding_61": -0.28380868, "title+abstract_embedding_62": 0.058382936, "title+abstract_embedding_63": -0.18913928, "title+abstract_embedding_64": -0.28338227, "title+abstract_embedding_65": -0.13446173, "title+abstract_embedding_66": -0.000208016, "title+abstract_embedding_67": 0.002578795, "title+abstract_embedding_68": 0.07435128, "title+abstract_embedding_69": 0.082548514, "title+abstract_embedding_70": 0.31416243, "title+abstract_embedding_71": -0.053252578, "title+abstract_embedding_72": -0.22445148, "title+abstract_embedding_73": -0.066566534, "title+abstract_embedding_74": -0.086598724, "title+abstract_embedding_75": -0.0301506, "title+abstract_embedding_76": 0.06744993, "title+abstract_embedding_77": -0.19806753, "title+abstract_embedding_78": 0.031122312, "title+abstract_embedding_79": 0.20329158, "title+abstract_embedding_80": 0.019840814, "title+abstract_embedding_81": -0.12779304, "title+abstract_embedding_82": -0.117907465, "title+abstract_embedding_83": -0.005416445, "title+abstract_embedding_84": -0.15657707, "title+abstract_embedding_85": -0.019262211, "title+abstract_embedding_86": -0.16986316, "title+abstract_embedding_87": 0.27855626, "title+abstract_embedding_88": 0.038124144, "title+abstract_embedding_89": 0.12880637, "title+abstract_embedding_90": -0.007186674, "title+abstract_embedding_91": 0.04639987, "title+abstract_embedding_92": 0.039902776, "title+abstract_embedding_93": 0.06699125, "title+abstract_embedding_94": 0.009712063, "title+abstract_embedding_95": -0.10210219, "title+abstract_embedding_96": -0.03304795, "title+abstract_embedding_97": 0.111534536, "title+abstract_embedding_98": 0.038188525, "title+abstract_embedding_99": -0.01724016, "title+abstract_embedding_100": -0.002531424, "title+abstract_embedding_101": -0.11377141, "title+abstract_embedding_102": 0.000305731, "title+abstract_embedding_103": -0.14208871, "title+abstract_embedding_104": 0.09913754, "title+abstract_embedding_105": -0.12770492, "title+abstract_embedding_106": 0.06562267, "title+abstract_embedding_107": 0.13653831, "title+abstract_embedding_108": -0.072041415, "title+abstract_embedding_109": 0.012747765, "title+abstract_embedding_110": -0.2662319, "title+abstract_embedding_111": -0.026706634, "title+abstract_embedding_112": 0.052820176, "title+abstract_embedding_113": 0.09053397, "title+abstract_embedding_114": 0.029541299, "title+abstract_embedding_115": 0.07187359, "title+abstract_embedding_116": 0.102560654, "title+abstract_embedding_117": -0.027994618, "title+abstract_embedding_118": 0.002708607, "title+abstract_embedding_119": 0.1210241, "title+abstract_embedding_120": -0.003857931, "title+abstract_embedding_121": -0.07502255, "title+abstract_embedding_122": -0.12563494, "title+abstract_embedding_123": -0.15117875, "title+abstract_embedding_124": 0.06482972, "title+abstract_embedding_125": 0.031328652, "title+abstract_embedding_126": 0.082053095, "title+abstract_embedding_127": 0.061184473, "label": 106, "label-multi": NaN }, { "paper_new_id": 96, "id": "j_74e479cf93e5788170d5527927e69331", "title+abstract": "Kinetics and initial photocatalytic pathway of tryptophan, important constituent of microorganisms;Abstract The adsorption equilibrium in the dark and under UV light, the kinetic of photocatalytic oxidation and the main initial pathways of tryptophan photocatalytic degradation has been investigated in aerated TiO 2 Degussa P-25 aqueous suspensions illuminated at |? ?>?340?nm. Tryptophan has been chosen as a model of organic compounds of amino acids, elemental constituents of DNA, microorganisms, e.g. bacteria, fungi, virus among others to better understand their photocatalytic degradation. Langmuir and Langmuir¡§CHinshelwood models have been used to determine the adsorption, the rate constants and the surface coverage of TiO 2 . Despite a low coverage of the TiO 2 surface in the dark a high photocatalytic degradability and initial mineralization occurred. However, the surface coverage of TiO 2 was about doubled under UV light suggesting the formation of active sites under irradiation. LC¡§CMS, LC¡§CUV with or without derivatization analyses allowed us to identify, mono-, di- and tri-hydroxylated compounds, deamination of heterocycle, the formation of six organic acid, oxalic, oxamique, lactic, formic, acetic and propanoic acids and of three linear amino acids, serine, aspartic acid and glycine. A degradation mechanism is proposed to the formation of oxamic acid. The study of the mineralization of carbon and nitrogen showed the presence of trace of organic molecules mineralizable with difficulty. Nitrogen atoms were predominantly photoconverted into NH 4 + . After more than 95% of carbon mineralization, NH 4 + /NO 3 ? ratio was 4. The identification of the photocatalytic products, their evolution and the TOC evolution indicated three initial competitive pathways: about 50% of hydroxylation with 6¡§C7% of the hydroxylation of carbon bearing NH 2 and COO ? , about 30% of decarboxylation and less than 20% of nitrogen¡§Ccarbon (N¡§CC) cleavage.", "title+abstract_embedding_0": 0.92415535, "title+abstract_embedding_1": 0.3769213, "title+abstract_embedding_2": 1.0668806, "title+abstract_embedding_3": -0.2433995, "title+abstract_embedding_4": 0.038941562, "title+abstract_embedding_5": -0.07237655, "title+abstract_embedding_6": -0.38284555, "title+abstract_embedding_7": 0.4334003, "title+abstract_embedding_8": -0.52878547, "title+abstract_embedding_9": -0.2636121, "title+abstract_embedding_10": 0.32574004, "title+abstract_embedding_11": -0.21252988, "title+abstract_embedding_12": -0.042236894, "title+abstract_embedding_13": 0.2673731, "title+abstract_embedding_14": 0.33470115, "title+abstract_embedding_15": 0.31184655, "title+abstract_embedding_16": 0.22410882, "title+abstract_embedding_17": 0.062083334, "title+abstract_embedding_18": -0.11002871, "title+abstract_embedding_19": 0.33862716, "title+abstract_embedding_20": -0.23758605, "title+abstract_embedding_21": -0.5466844, "title+abstract_embedding_22": -0.28001386, "title+abstract_embedding_23": -0.21341336, "title+abstract_embedding_24": -0.18157601, "title+abstract_embedding_25": 0.00266844, "title+abstract_embedding_26": -0.26860458, "title+abstract_embedding_27": 0.11191334, "title+abstract_embedding_28": 0.16525266, "title+abstract_embedding_29": -0.075500265, "title+abstract_embedding_30": -0.11466725, "title+abstract_embedding_31": -0.28365636, "title+abstract_embedding_32": -0.084088154, "title+abstract_embedding_33": -0.03223078, "title+abstract_embedding_34": -0.20063016, "title+abstract_embedding_35": -0.30048043, "title+abstract_embedding_36": 0.07434216, "title+abstract_embedding_37": 0.184602, "title+abstract_embedding_38": -0.1404125, "title+abstract_embedding_39": -0.38172683, "title+abstract_embedding_40": 0.03001383, "title+abstract_embedding_41": 0.11545156, "title+abstract_embedding_42": -0.078244895, "title+abstract_embedding_43": -0.040097743, "title+abstract_embedding_44": 0.14768998, "title+abstract_embedding_45": -0.076907575, "title+abstract_embedding_46": -0.137645, "title+abstract_embedding_47": -0.057096258, "title+abstract_embedding_48": -0.114529744, "title+abstract_embedding_49": 0.09206922, "title+abstract_embedding_50": 0.09506415, "title+abstract_embedding_51": 0.18012401, "title+abstract_embedding_52": -0.019398294, "title+abstract_embedding_53": 0.13274893, "title+abstract_embedding_54": -0.13041237, "title+abstract_embedding_55": -0.12314786, "title+abstract_embedding_56": -0.06161926, "title+abstract_embedding_57": -0.13164318, "title+abstract_embedding_58": 0.2055118, "title+abstract_embedding_59": 0.0858112, "title+abstract_embedding_60": -0.012705445, "title+abstract_embedding_61": -0.21590179, "title+abstract_embedding_62": -0.27634212, "title+abstract_embedding_63": -0.07697566, "title+abstract_embedding_64": -0.069370955, "title+abstract_embedding_65": -0.023192883, "title+abstract_embedding_66": -0.004293736, "title+abstract_embedding_67": -0.2273435, "title+abstract_embedding_68": -0.090486206, "title+abstract_embedding_69": 0.12196424, "title+abstract_embedding_70": -0.025312059, "title+abstract_embedding_71": -0.002080485, "title+abstract_embedding_72": 0.022135189, "title+abstract_embedding_73": 0.16900253, "title+abstract_embedding_74": 0.028774701, "title+abstract_embedding_75": -0.021083802, "title+abstract_embedding_76": -0.020169467, "title+abstract_embedding_77": -0.14439501, "title+abstract_embedding_78": -0.074747704, "title+abstract_embedding_79": 0.25741497, "title+abstract_embedding_80": 0.15321493, "title+abstract_embedding_81": -0.025468707, "title+abstract_embedding_82": -0.13506061, "title+abstract_embedding_83": -0.25431138, "title+abstract_embedding_84": -0.00952372, "title+abstract_embedding_85": -0.04565511, "title+abstract_embedding_86": -0.11543239, "title+abstract_embedding_87": 0.1614168, "title+abstract_embedding_88": -0.0674799, "title+abstract_embedding_89": 0.025327466, "title+abstract_embedding_90": -0.23204425, "title+abstract_embedding_91": -0.14761898, "title+abstract_embedding_92": -0.07095049, "title+abstract_embedding_93": -0.08028455, "title+abstract_embedding_94": -0.07856953, "title+abstract_embedding_95": -0.0743555, "title+abstract_embedding_96": -0.077514626, "title+abstract_embedding_97": -0.08617835, "title+abstract_embedding_98": 0.000916492, "title+abstract_embedding_99": -0.0229806, "title+abstract_embedding_100": 0.1273654, "title+abstract_embedding_101": 0.03580694, "title+abstract_embedding_102": 0.06694555, "title+abstract_embedding_103": -0.005207107, "title+abstract_embedding_104": -0.112214625, "title+abstract_embedding_105": 0.12995517, "title+abstract_embedding_106": 0.052498654, "title+abstract_embedding_107": -0.1548244, "title+abstract_embedding_108": 0.021987617, "title+abstract_embedding_109": 0.10642545, "title+abstract_embedding_110": -0.05605237, "title+abstract_embedding_111": -0.022875331, "title+abstract_embedding_112": -0.065824494, "title+abstract_embedding_113": -0.027102038, "title+abstract_embedding_114": -0.06501315, "title+abstract_embedding_115": 0.08041257, "title+abstract_embedding_116": 0.07461702, "title+abstract_embedding_117": 0.15890788, "title+abstract_embedding_118": -0.11946299, "title+abstract_embedding_119": -0.09486146, "title+abstract_embedding_120": -0.04802344, "title+abstract_embedding_121": 0.053827927, "title+abstract_embedding_122": 0.11200175, "title+abstract_embedding_123": 0.011871412, "title+abstract_embedding_124": -0.055433743, "title+abstract_embedding_125": -0.03260293, "title+abstract_embedding_126": -0.033890985, "title+abstract_embedding_127": 0.10262669, "label": 3, "label-multi": "0;3" }, { "paper_new_id": 97, "id": "j_78ed0186b8a8136a6bb903c0bd1f3ca4", "title+abstract": "Photooxidation of iodide ion on some semiconductor and non-semiconductor surfaces;Abstract In 80% aqueous ethanol, TiO2 (anatase), ZrO2, ZnO, V2O5, Fe2O3 and Al2O3 photocatalyze the oxidation of iodide ion but CdO and CdS do not; the wavelength of illumination is 365 nm. However, Fe2O3 fails to bring in a sustainable photocatalysis in 60% aqueous ethanol. The photooxidation of iodide ion on TiO2, ZrO2, ZnO, V2O5 and Al2O3 in 60% aqueous ethanol was studied as a function of I?], amount of catalyst suspended, airflow rate, light intensity and solvent composition. The metal oxides examined show sustainable photocatalytic activity. Iodine formation is larger with illumination at 254 nm than at 365 nm. The mechanisms of photocatalysis on semiconductor and non-semiconductor surfaces have been discussed. Photocatalytic generation of iodine has been analyzed using a kinetic model. The photocatalytic efficiencies are of the order V2O5?>?TiO2?>?ZrO2?>?ZnO?>?Al2O3 and V2O5?>?TiO2?>?ZrO2?>?ZnO=Fe2O3?>?Al2O3 in 60% and 80% aqueous ethanol.", "title+abstract_embedding_0": 0.5659337, "title+abstract_embedding_1": 0.63515455, "title+abstract_embedding_2": 0.5140696, "title+abstract_embedding_3": -0.27414668, "title+abstract_embedding_4": 0.48766142, "title+abstract_embedding_5": -0.30725378, "title+abstract_embedding_6": 0.41834265, "title+abstract_embedding_7": -0.14400281, "title+abstract_embedding_8": -0.15047947, "title+abstract_embedding_9": -0.50892115, "title+abstract_embedding_10": 0.6112258, "title+abstract_embedding_11": 0.14006814, "title+abstract_embedding_12": 0.014350191, "title+abstract_embedding_13": 0.003282111, "title+abstract_embedding_14": 0.22699231, "title+abstract_embedding_15": -0.064761184, "title+abstract_embedding_16": -0.026768118, "title+abstract_embedding_17": 0.48617753, "title+abstract_embedding_18": 0.35040635, 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"title+abstract_embedding_109": 0.09439851, "title+abstract_embedding_110": -0.18280387, "title+abstract_embedding_111": -0.016237358, "title+abstract_embedding_112": -0.09788044, "title+abstract_embedding_113": -0.06074229, "title+abstract_embedding_114": 0.18263304, "title+abstract_embedding_115": -0.08552375, "title+abstract_embedding_116": -0.10443291, "title+abstract_embedding_117": -0.03150347, "title+abstract_embedding_118": 0.059446536, "title+abstract_embedding_119": 0.13273542, "title+abstract_embedding_120": 0.04835746, "title+abstract_embedding_121": 0.036826216, "title+abstract_embedding_122": 0.045842767, "title+abstract_embedding_123": -0.14227675, "title+abstract_embedding_124": 0.034415916, "title+abstract_embedding_125": 0.18140772, "title+abstract_embedding_126": 0.18874088, "title+abstract_embedding_127": -0.10747576, "label": 3, "label-multi": "3" }, { "paper_new_id": 98, "id": "j_7d612d00179133e881effff848ae88b3", "title+abstract": "Gold Nanoparticles Doped Conducting Polymer Nanorod Electrodes: Ferrocene Catalyzed Aptamer-Based Thrombin Immunosensor;Au nanoparticles-doped conducting polymer nanorods electrodes (AuNPs/CPNEs) were prepared by coating Au nanorods (AuNRs) with a conducting polymer layer. The AuNRs were prepared through an electroless deposition method using the polycarbonate membrane (pore diameter, 50 nm, pore density, 6 x 10(8) pores/cm(2)) as a template. The AuNPs/CPNEs combining catalytic activity of ferrocene to ascorbic acid were used for the fabrication of an ultrasensitive aptamer sensor for thrombin detection. The AuNPs/3D-CPNEs were characterized employing cyclic voltammetry (CV), X-ray photoelectron spectroscopy (XPS), scanning electron microscopy (SEM), and atomic force microscopy (AFM). Sandwiched immunoassay for alpha-human thrombin with NH(2)-functionalized-thrombin binding aptamer (Apt) immobilized on AuNPs/3D-CPNEs was studied through the electrocatalytic oxidation of ascorbic acid by the ferrocene moiety that was bound with an antithrombin antibody and attached with the Apt/3D-CPNEs probe through target binding. Various experimental parameters affecting thrombin detection were optimized, and the performance of the thrombin aptamer sensor was examined. The Apt/AuNPs/3D-CPNEs based thrombin sensor exhibited a wide dynamic range of 5-2000 ng L(-1) and a low detection limit of 5 ng L(-1) (0.14 pM). The selectivity and the stability of the proposed thrombin aptamer sensor were excellent, and it was tested in a real human serum sample for the detection of spiked concentrations of thrombin.", "title+abstract_embedding_0": 0.8460201, "title+abstract_embedding_1": -1.1291094, "title+abstract_embedding_2": -0.20727542, "title+abstract_embedding_3": 0.24772304, "title+abstract_embedding_4": -0.56514823, "title+abstract_embedding_5": -0.004245877, "title+abstract_embedding_6": -0.59024894, "title+abstract_embedding_7": 0.37259328, "title+abstract_embedding_8": -0.13399555, "title+abstract_embedding_9": -0.23034078, "title+abstract_embedding_10": 0.27981955, "title+abstract_embedding_11": 0.400331, "title+abstract_embedding_12": 0.007260189, "title+abstract_embedding_13": 0.06560563, "title+abstract_embedding_14": -0.3055405, "title+abstract_embedding_15": -0.02397319, "title+abstract_embedding_16": -0.030989558, "title+abstract_embedding_17": -0.03143683, "title+abstract_embedding_18": 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"title+abstract_embedding_109": 0.12544869, "title+abstract_embedding_110": 0.14604333, "title+abstract_embedding_111": -0.20964089, "title+abstract_embedding_112": -0.04511489, "title+abstract_embedding_113": -0.19996817, "title+abstract_embedding_114": -0.046203822, "title+abstract_embedding_115": 0.014339112, "title+abstract_embedding_116": 0.113638535, "title+abstract_embedding_117": 0.0419838, "title+abstract_embedding_118": -0.0287611, "title+abstract_embedding_119": 0.09814751, "title+abstract_embedding_120": 0.056599196, "title+abstract_embedding_121": -0.017300086, "title+abstract_embedding_122": 0.017856687, "title+abstract_embedding_123": 0.008270048, "title+abstract_embedding_124": -0.06906041, "title+abstract_embedding_125": 0.18389535, "title+abstract_embedding_126": 0.041262567, "title+abstract_embedding_127": 0.09026093, "label": 106, "label-multi": NaN }, { "paper_new_id": 99, "id": "j_7e79e98ea90285f156c52d82fe3ee669", "title+abstract": "Photocatalytic activity of TiO2a??SiO2 nanocomposites applied to buildings: Influence of particle size and loading;Atmospheric pollution has an evidently adverse impact on the esthetics of urban buildings and structures. Thus, the synthesis of photocatalysts capable of removing pollutants deposited on the surface of stone and other building materials is a challenge to researchers. By a simple and low cost process we have synthesized mesoporous TiO2¡§CSiO2 photocatalytic coatings that meet the requirements of outdoor application. These are new materials designed to give to the building material long-term self-cleaning and strengthening properties. \n \nWe have varied the loading and size of TiO2 nanoparticles in order to investigate their effect on the photocatalytic activity. We find that the integration of larger and sharper titania particles in a silica network with a titania content of around 4% (w/v) significantly improves self-cleaning effectiveness, due to the enhanced availability of surface photoactive sites. For a higher TiO2 content (10%, w/v), photocatalytic action decreases because the porous volume is drastically reduced and consequently, access to photoactive sites is more difficult.", "title+abstract_embedding_0": 0.03976202, "title+abstract_embedding_1": 1.133036, "title+abstract_embedding_2": -0.2682512, "title+abstract_embedding_3": 0.8111171, "title+abstract_embedding_4": 0.35994524, "title+abstract_embedding_5": 0.5692696, "title+abstract_embedding_6": -0.20991305, "title+abstract_embedding_7": -0.18251944, "title+abstract_embedding_8": -0.08035274, "title+abstract_embedding_9": 0.10487768, "title+abstract_embedding_10": -0.18053326, "title+abstract_embedding_11": -0.17925268, "title+abstract_embedding_12": 0.34842086, "title+abstract_embedding_13": 0.2068617, "title+abstract_embedding_14": 0.02099225, "title+abstract_embedding_15": -0.10367576, "title+abstract_embedding_16": -0.20635702, "title+abstract_embedding_17": 0.08664632, "title+abstract_embedding_18": -0.37564552, 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"title+abstract_embedding_87": 0.008940626, "title+abstract_embedding_88": -0.027157664, "title+abstract_embedding_89": 0.08457567, "title+abstract_embedding_90": -0.06981809, "title+abstract_embedding_91": 0.112997875, "title+abstract_embedding_92": 0.13706116, "title+abstract_embedding_93": -0.11784481, "title+abstract_embedding_94": -0.09096808, "title+abstract_embedding_95": 0.20423627, "title+abstract_embedding_96": 0.032381415, "title+abstract_embedding_97": -0.009599772, "title+abstract_embedding_98": -0.20201991, "title+abstract_embedding_99": -0.09460437, "title+abstract_embedding_100": 0.033988878, "title+abstract_embedding_101": 0.16103278, "title+abstract_embedding_102": 0.08621389, "title+abstract_embedding_103": 0.027720168, "title+abstract_embedding_104": -0.12749177, "title+abstract_embedding_105": -0.030092746, "title+abstract_embedding_106": -0.049676195, "title+abstract_embedding_107": 0.053029053, "title+abstract_embedding_108": -0.006694637, "title+abstract_embedding_109": -0.02736482, "title+abstract_embedding_110": 0.20594108, "title+abstract_embedding_111": 0.13767329, "title+abstract_embedding_112": -0.016755983, "title+abstract_embedding_113": 0.03422942, "title+abstract_embedding_114": 0.10693875, "title+abstract_embedding_115": 0.024104446, "title+abstract_embedding_116": -0.17264052, "title+abstract_embedding_117": 0.05041246, "title+abstract_embedding_118": -0.07095479, "title+abstract_embedding_119": -0.047725033, "title+abstract_embedding_120": -0.046119794, "title+abstract_embedding_121": -0.029017607, "title+abstract_embedding_122": 0.01389268, "title+abstract_embedding_123": -0.13571708, "title+abstract_embedding_124": -0.15315339, "title+abstract_embedding_125": 0.1659536, "title+abstract_embedding_126": -0.15198064, "title+abstract_embedding_127": 0.10231565, "label": 3, "label-multi": "0;3" }, { "paper_new_id": 100, "id": "j_7ed0c27dfc699ceb5d1ad94579ba597b", "title+abstract": "Hierarchical architectures of ZnSa??In2S3 solid solution onto TiO2 nanofibers with high visible-light photocatalytic activity;A unique hierarchical architecture of ZnS-In2S3 solid solution nanostructures onto TiO2 nanofibers (TiO2@ZnS-In2S3) has been successfully fabricated by simple hydrothermal method. The ZnS-In2S3 solid solution nanostructures exhibit a diversity of morphologies: nanosheet, nanorod and nanoparticle. The porous TiO2 nanofiber templates effectively inhibit the aggregation growth of ZnS-In2S3 solid solution. The formation of ZnS-In2S3 solid solution is proved by X-ray diffraction (XRD) and X-ray photoelectron spectroscopy (XPS) and the intimate contact between TiO2 nanofibers and ZnS-In2S3 solid solution favors fast transfer of photogenerated electrons. The trinary TiO2@ZnS-In2S3 heterostructures exhibit high adsorption capacity and visible light photocatalytic activity for the degradation of rhodamine B dye (RhB), remarkably superior to pure TiO2 nanofibers or binary structures (ZnS/TiO2 nanofibers, In2S3/TiO2 nanofibers and ZnS-In2S3 solid solution). Under visible light irradiation the RhB photocatalytic degradation rate over TiO2@ZnS-In2S3 heterostructures is about 16.7, 12.5, 6.3, 5.9, and 2.2 times that over pure TiO2 nanofibers, ZnS nanoparticles, In2S3/TiO2 nanofibers, ZnS/TiO2 nanofibers, and ZnS-In2S3 solid solution, respectively. Furthermore, the TiO2@ZnS-In2S3 heterostructures show highly stable recycling performance. (C) 2014 Elsevier B. V. All rights reserved.", "title+abstract_embedding_0": 1.2989317, "title+abstract_embedding_1": 0.0406197, "title+abstract_embedding_2": -1.2522308, "title+abstract_embedding_3": -0.21309209, "title+abstract_embedding_4": 0.420461, "title+abstract_embedding_5": -0.35353953, "title+abstract_embedding_6": -0.14778486, "title+abstract_embedding_7": 0.37096784, "title+abstract_embedding_8": -0.2841018, "title+abstract_embedding_9": 0.4363927, "title+abstract_embedding_10": -0.6452557, "title+abstract_embedding_11": -0.37136927, "title+abstract_embedding_12": 0.4857519, "title+abstract_embedding_13": -0.03138507, "title+abstract_embedding_14": 0.019080222, "title+abstract_embedding_15": -0.25502846, "title+abstract_embedding_16": -0.01955846, "title+abstract_embedding_17": -0.5312037, "title+abstract_embedding_18": 0.004090548, "title+abstract_embedding_19": 0.1865238, "title+abstract_embedding_20": 0.18317966, "title+abstract_embedding_21": -0.21990663, "title+abstract_embedding_22": 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"title+abstract_embedding_112": 0.07334748, "title+abstract_embedding_113": 0.040693358, "title+abstract_embedding_114": 0.095541924, "title+abstract_embedding_115": -0.19297406, "title+abstract_embedding_116": -0.12569226, "title+abstract_embedding_117": 0.12095104, "title+abstract_embedding_118": 0.059638742, "title+abstract_embedding_119": 0.12019825, "title+abstract_embedding_120": -0.030753085, "title+abstract_embedding_121": 0.09276832, "title+abstract_embedding_122": 0.12009123, "title+abstract_embedding_123": -0.05455802, "title+abstract_embedding_124": 0.039169118, "title+abstract_embedding_125": 0.21863782, "title+abstract_embedding_126": 0.018215869, "title+abstract_embedding_127": 0.08615711, "label": 3, "label-multi": "1;18;3" }, { "paper_new_id": 101, "id": "j_7f63cba2359dac118668cdd81065f8a0", "title+abstract": "A novel method for photodegradation of high-chroma dye wastewater via electrochemical pre-oxidation;A new two-step process involving the electrocatalytic (EC) pre-oxidation and the following photoelectrocatalytic synergistic (PEC) oxidation is proposed to treat the high concentration and high-chroma methyl orange dye wastewater, which cannot be degraded by photocatalytic oxidation (PC) directly. The SnO(2)/TiO(2)-NTs/Ti electrode simultaneously possessing the outstanding PC oxidation properties of TiO(2)-NTs and the excellent EC oxidation abilities of the Sb doped SnO(2) was synthesized by impregnating Sb doped SnO(2) nanoparticles into TiO(2)-NTs. In the pre-oxidation process as the first stage, the high-color dye wastewater is decolorized with electrochemical method to some extent. Then, the wastewater becomes a light transmission system. It provides a suitable condition for PC oxidation reaction in the second stage. The synergistic effects of PC and EC oxidation led to the high PEC efficiency and the complete mineralization of dye wastewater is achieved. This two-step process is fast and efficient, which is worthy to study and explore in the practical environmental treatment.", "title+abstract_embedding_0": -0.075062275, "title+abstract_embedding_1": 0.22549188, "title+abstract_embedding_2": 0.44578838, "title+abstract_embedding_3": 0.43682694, "title+abstract_embedding_4": 0.28798598, "title+abstract_embedding_5": -0.41533685, "title+abstract_embedding_6": -0.45278594, "title+abstract_embedding_7": 0.031612746, "title+abstract_embedding_8": -0.016961642, "title+abstract_embedding_9": 0.020790398, "title+abstract_embedding_10": -0.008072779, "title+abstract_embedding_11": 0.43925634, "title+abstract_embedding_12": 0.15936652, "title+abstract_embedding_13": 0.043749504, "title+abstract_embedding_14": -0.093153015, "title+abstract_embedding_15": -0.030658867, "title+abstract_embedding_16": -0.2105112, "title+abstract_embedding_17": -0.24952115, "title+abstract_embedding_18": 0.4309339, "title+abstract_embedding_19": -0.20361565, 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"title+abstract_embedding_111": 0.034666054, "title+abstract_embedding_112": -0.18599011, "title+abstract_embedding_113": -0.04945208, "title+abstract_embedding_114": -0.14893794, "title+abstract_embedding_115": -0.06759945, "title+abstract_embedding_116": 0.005140379, "title+abstract_embedding_117": -0.03599754, "title+abstract_embedding_118": -0.11649882, "title+abstract_embedding_119": 0.000896237, "title+abstract_embedding_120": -0.2412571, "title+abstract_embedding_121": 0.07073129, "title+abstract_embedding_122": -0.044246405, "title+abstract_embedding_123": -0.062239304, "title+abstract_embedding_124": 0.020512149, "title+abstract_embedding_125": 0.025417946, "title+abstract_embedding_126": 0.06431741, "title+abstract_embedding_127": 0.16274357, "label": 16, "label-multi": "16" }, { "paper_new_id": 102, "id": "j_80b548caf08f1f9cc50ea45dc26b8945", "title+abstract": "Arylene Ethynylene-Functionalized Bithiazole-Based Zinc Polymers for Ultraefficient Photocatalytic Activity;Polymers 4 containing poly(arylene ethynylene) were synthesized and characterized systematically. Among them, 4c exhibited a remarkable H2 evolution rate.(14.32 mmol h?1 g?1) with visible-light irradiation, lasting 72 h in different water qualities; the corresponding apparent quantum yield was 11.6% at 450 nm..", "title+abstract_embedding_0": -1.0447485, "title+abstract_embedding_1": 0.7470275, "title+abstract_embedding_2": 0.16867715, "title+abstract_embedding_3": 0.1699422, "title+abstract_embedding_4": -0.7812611, "title+abstract_embedding_5": -0.34618855, "title+abstract_embedding_6": 0.5640858, "title+abstract_embedding_7": 0.1924826, "title+abstract_embedding_8": 0.6267987, "title+abstract_embedding_9": 0.4025094, "title+abstract_embedding_10": 0.13346852, "title+abstract_embedding_11": -0.5087799, "title+abstract_embedding_12": -0.07595718, "title+abstract_embedding_13": -0.13794091, "title+abstract_embedding_14": 0.18453023, "title+abstract_embedding_15": -0.036574684, "title+abstract_embedding_16": -0.030030102, "title+abstract_embedding_17": 0.12587681, 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"title+abstract_embedding_109": -0.09556326, "title+abstract_embedding_110": 0.20241341, "title+abstract_embedding_111": 0.022623986, "title+abstract_embedding_112": -0.09498958, "title+abstract_embedding_113": 0.07921439, "title+abstract_embedding_114": 0.024212986, "title+abstract_embedding_115": 0.14775051, "title+abstract_embedding_116": -0.088111326, "title+abstract_embedding_117": 0.13283041, "title+abstract_embedding_118": -0.031426765, "title+abstract_embedding_119": 0.061537746, "title+abstract_embedding_120": 0.104134634, "title+abstract_embedding_121": 0.05867646, "title+abstract_embedding_122": -0.025736481, "title+abstract_embedding_123": -0.17970094, "title+abstract_embedding_124": 0.022626556, "title+abstract_embedding_125": 0.23446596, "title+abstract_embedding_126": -0.04956273, "title+abstract_embedding_127": 0.26247957, "label": 3, "label-multi": "3" }, { "paper_new_id": 103, "id": "j_8232ec72575b81910af0370b92ad5df8", "title+abstract": "LaTiO2N as a Visible-Light (a??¨¨600 nm)-Driven Photocatalyst (2);LaTiO2N, a Ti-based oxynitride, was studied as a visible-light (420?600 nm)-driven photocatalyst. DFT calculation for LaTiO2N indicated that the top of the valence band consists predominantly of N 2p orbitals with a small contribution by O 2p orbitals, while the bottom of the conduction band is made up entirely of empty Ti 3d orbitals. LaTiO2N was synthesized from a La2Ti2O7 precursor at 1123 K under NH3 flow. The relationship between the preparation condition and the photocatalytic activities of H+ reduction to H2 and H2O oxidation to O2 was examined. It was found that the photocatalytic activity for O2 evolution increased with nitridation time, reaching a maximum at 72 h. Further treatment beyond 72 h lowered the rate of O2 evolution. The rate of H2 evolution was almost independent of nitridation time. The relationship between nitridation time and the rate of O2 evolution is discussed on the basis of X-ray photoelectron spectroscopy (XPS) analyses.", "title+abstract_embedding_0": 0.4876392, "title+abstract_embedding_1": 0.85853446, "title+abstract_embedding_2": 0.44013724, "title+abstract_embedding_3": -0.109946966, "title+abstract_embedding_4": 0.6625331, "title+abstract_embedding_5": 0.13297492, "title+abstract_embedding_6": 0.526663, "title+abstract_embedding_7": -0.19391075, "title+abstract_embedding_8": -0.30622524, "title+abstract_embedding_9": 0.6729805, "title+abstract_embedding_10": 0.61887634, "title+abstract_embedding_11": -0.2318934, "title+abstract_embedding_12": 0.20762599, "title+abstract_embedding_13": 0.12763572, "title+abstract_embedding_14": -0.18917304, "title+abstract_embedding_15": -0.10659681, "title+abstract_embedding_16": 0.34195763, "title+abstract_embedding_17": 0.037504107, "title+abstract_embedding_18": 0.1658947, "title+abstract_embedding_19": 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-0.043689847, "title+abstract_embedding_43": 0.04532163, "title+abstract_embedding_44": 0.19223751, "title+abstract_embedding_45": 0.15872878, "title+abstract_embedding_46": 0.08921319, "title+abstract_embedding_47": -0.06292008, "title+abstract_embedding_48": -0.032920063, "title+abstract_embedding_49": 0.3196802, "title+abstract_embedding_50": -0.27939317, "title+abstract_embedding_51": 0.029709369, "title+abstract_embedding_52": 0.043744415, "title+abstract_embedding_53": -0.09952557, "title+abstract_embedding_54": 0.22716533, "title+abstract_embedding_55": 0.2587786, "title+abstract_embedding_56": -0.14795767, "title+abstract_embedding_57": -0.05179511, "title+abstract_embedding_58": 0.13207395, "title+abstract_embedding_59": -0.220582, "title+abstract_embedding_60": 0.15903491, "title+abstract_embedding_61": -0.256477, "title+abstract_embedding_62": 0.11188914, "title+abstract_embedding_63": 0.08365183, "title+abstract_embedding_64": -0.21579383, "title+abstract_embedding_65": -0.28915793, "title+abstract_embedding_66": -0.15261579, "title+abstract_embedding_67": -0.3378942, "title+abstract_embedding_68": -0.072564535, "title+abstract_embedding_69": 0.17780446, "title+abstract_embedding_70": -0.2185975, "title+abstract_embedding_71": 0.024410129, "title+abstract_embedding_72": 0.047375403, "title+abstract_embedding_73": -0.17632361, "title+abstract_embedding_74": 0.04566118, "title+abstract_embedding_75": 0.02471203, "title+abstract_embedding_76": 0.031441867, "title+abstract_embedding_77": 0.33839518, "title+abstract_embedding_78": 0.074816674, "title+abstract_embedding_79": 0.016939804, "title+abstract_embedding_80": -0.001925398, "title+abstract_embedding_81": -0.19007203, "title+abstract_embedding_82": 0.2823576, "title+abstract_embedding_83": 0.032828465, "title+abstract_embedding_84": 0.000951603, "title+abstract_embedding_85": -0.027761871, "title+abstract_embedding_86": -0.07171122, "title+abstract_embedding_87": -0.09963112, "title+abstract_embedding_88": 0.05079706, "title+abstract_embedding_89": -0.006827794, "title+abstract_embedding_90": 0.034583524, "title+abstract_embedding_91": 0.11028084, "title+abstract_embedding_92": 0.017983392, "title+abstract_embedding_93": 0.034503095, "title+abstract_embedding_94": -0.069276705, "title+abstract_embedding_95": -0.202562, "title+abstract_embedding_96": 0.081423864, "title+abstract_embedding_97": 0.08720668, "title+abstract_embedding_98": 0.13196097, "title+abstract_embedding_99": 0.06765402, "title+abstract_embedding_100": 0.051059358, "title+abstract_embedding_101": -0.01656324, "title+abstract_embedding_102": -0.11669484, "title+abstract_embedding_103": 0.1548379, "title+abstract_embedding_104": -0.04652764, "title+abstract_embedding_105": 0.11773022, "title+abstract_embedding_106": -0.057021737, "title+abstract_embedding_107": 0.07900899, "title+abstract_embedding_108": 0.08160111, "title+abstract_embedding_109": 0.050236955, "title+abstract_embedding_110": 0.11331728, "title+abstract_embedding_111": -0.060600802, "title+abstract_embedding_112": -0.03538713, "title+abstract_embedding_113": -0.2963339, "title+abstract_embedding_114": -0.026284307, "title+abstract_embedding_115": 0.08614316, "title+abstract_embedding_116": -0.21317074, "title+abstract_embedding_117": -0.04835853, "title+abstract_embedding_118": -0.14821318, "title+abstract_embedding_119": 0.13266547, "title+abstract_embedding_120": -0.029909018, "title+abstract_embedding_121": -0.037326053, "title+abstract_embedding_122": 0.032994375, "title+abstract_embedding_123": -0.000584446, "title+abstract_embedding_124": 0.04215853, "title+abstract_embedding_125": 0.069517285, "title+abstract_embedding_126": -0.05087719, "title+abstract_embedding_127": 0.052513547, "label": 3, "label-multi": "3" }, { "paper_new_id": 104, "id": "j_82b896e15f21adeafdd6fd50bdd3d2ec", "title+abstract": "Supera??Exchange Interaction Induced Overall Optimization in Ferromagnetic Perovskite Oxides Enables Ultrafast Water Oxidation;Oxygen evolution reaction (OER) is crucial in many renewable electrochemical technologies including regenerative fuel cells, rechargeable metal-air batteries, and water splitting. It is found that abundant active sites with favorable electronic structure and high electrical conductivity play a dominant role in achieving high electrocatalytic efficiency of perovskites, thus efficient strategies need to be designed to generate multiple beneficial factors for OER. Here, highlighted is an unusual super-exchange effect in ferromagnetic perovskite oxide to optimize active sites and enhance electrical conductivity. A systematic exploration about the composition-dependent OER activity in SrCo1 x Rux O3- |? (denoted as SCRx) (x = 0.0-1.0) perovskite is displayed with special attention on the role of super-exchange interaction between high spin (HS) Co3+ and Ru5+ ions. Induced by the unique Co3+ -O-Ru5+ super-exchange interactions, the SCR0.1 is endowed with abundant OER active species including Co3+ /Co4+ , Ru5+ , and O2 2- /O- , high electrical conductivity, and metal-oxygen covalency. Benefiting from these advantageous factors for OER electrocatalysis, the optimized SCR0.1 catalyst exhibits a remarkable activity with a low overpotential of 360 mV at 10 mA cm-2 , which exceeds the benchmark RuO2 and most well-known perovskite oxides reported so far, while maintaining excellent durability. This work provides a new pathway in developing perovskite catalysts for efficient catalysis.", "title+abstract_embedding_0": 0.37150335, "title+abstract_embedding_1": -0.6619512, "title+abstract_embedding_2": 0.19236718, "title+abstract_embedding_3": -0.82780814, "title+abstract_embedding_4": 0.89253587, "title+abstract_embedding_5": 0.051453292, "title+abstract_embedding_6": 0.02224812, "title+abstract_embedding_7": -0.21769598, "title+abstract_embedding_8": -0.30946225, "title+abstract_embedding_9": 0.21874994, "title+abstract_embedding_10": -0.012261741, "title+abstract_embedding_11": 0.07823874, "title+abstract_embedding_12": 0.44665197, "title+abstract_embedding_13": 0.19637203, "title+abstract_embedding_14": -0.21245769, "title+abstract_embedding_15": -0.2189729, "title+abstract_embedding_16": -0.36104694, "title+abstract_embedding_17": -0.025598213, "title+abstract_embedding_18": 0.000383668, "title+abstract_embedding_19": -0.07938807, "title+abstract_embedding_20": -0.1552602, "title+abstract_embedding_21": 0.002822131, "title+abstract_embedding_22": 0.5289205, "title+abstract_embedding_23": 0.099977136, "title+abstract_embedding_24": 0.29700518, "title+abstract_embedding_25": -0.1930204, "title+abstract_embedding_26": -0.1733886, "title+abstract_embedding_27": 0.522793, "title+abstract_embedding_28": 0.028518423, "title+abstract_embedding_29": -0.5852254, "title+abstract_embedding_30": -0.24683492, "title+abstract_embedding_31": -0.15478638, "title+abstract_embedding_32": 0.06959109, "title+abstract_embedding_33": 0.18683667, "title+abstract_embedding_34": 0.26051095, "title+abstract_embedding_35": -0.058294967, "title+abstract_embedding_36": 0.07933375, "title+abstract_embedding_37": -0.35816553, "title+abstract_embedding_38": 0.00640709, "title+abstract_embedding_39": 0.09623332, "title+abstract_embedding_40": -0.05945766, "title+abstract_embedding_41": 0.12967221, "title+abstract_embedding_42": -0.12725866, "title+abstract_embedding_43": 0.19594328, "title+abstract_embedding_44": 0.2532373, "title+abstract_embedding_45": 0.002381057, "title+abstract_embedding_46": -0.14425129, "title+abstract_embedding_47": 0.048531156, "title+abstract_embedding_48": -0.14460608, "title+abstract_embedding_49": 0.1885238, "title+abstract_embedding_50": 0.001590096, "title+abstract_embedding_51": 0.01873976, "title+abstract_embedding_52": 0.089807704, "title+abstract_embedding_53": -0.055004463, "title+abstract_embedding_54": -0.045790985, "title+abstract_embedding_55": -0.0687601, "title+abstract_embedding_56": -0.09578001, "title+abstract_embedding_57": 0.027142912, "title+abstract_embedding_58": -0.26932466, "title+abstract_embedding_59": 0.2975281, "title+abstract_embedding_60": -0.0798046, "title+abstract_embedding_61": 0.023650683, "title+abstract_embedding_62": 0.017702518, "title+abstract_embedding_63": -0.0857816, "title+abstract_embedding_64": -0.01231806, "title+abstract_embedding_65": -0.22797768, "title+abstract_embedding_66": 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"title+abstract_embedding_89": 0.16880533, "title+abstract_embedding_90": 0.15105115, "title+abstract_embedding_91": -0.002090551, "title+abstract_embedding_92": -0.12696365, "title+abstract_embedding_93": 0.2376441, "title+abstract_embedding_94": -0.03053192, "title+abstract_embedding_95": 0.079464465, "title+abstract_embedding_96": -0.14716855, "title+abstract_embedding_97": -0.074279934, "title+abstract_embedding_98": 0.093627155, "title+abstract_embedding_99": -0.11662445, "title+abstract_embedding_100": -0.066681996, "title+abstract_embedding_101": 0.056790084, "title+abstract_embedding_102": -0.014229454, "title+abstract_embedding_103": -0.15092668, "title+abstract_embedding_104": 0.1813689, "title+abstract_embedding_105": -0.000295851, "title+abstract_embedding_106": 0.10797053, "title+abstract_embedding_107": 0.05818896, "title+abstract_embedding_108": -0.22080049, "title+abstract_embedding_109": 0.11761288, "title+abstract_embedding_110": -0.0964195, "title+abstract_embedding_111": 0.013391454, "title+abstract_embedding_112": 0.052367687, "title+abstract_embedding_113": 0.068329796, "title+abstract_embedding_114": 0.06618647, "title+abstract_embedding_115": 0.005589396, "title+abstract_embedding_116": -0.055869117, "title+abstract_embedding_117": -0.022609934, "title+abstract_embedding_118": 0.024758775, "title+abstract_embedding_119": 0.028360147, "title+abstract_embedding_120": -0.09269114, "title+abstract_embedding_121": -0.008998277, "title+abstract_embedding_122": 0.10478711, "title+abstract_embedding_123": -0.051990587, "title+abstract_embedding_124": 0.10798879, "title+abstract_embedding_125": 0.12433401, "title+abstract_embedding_126": 0.026558504, "title+abstract_embedding_127": -0.095855534, "label": 3, "label-multi": "1;15;2;3" }, { "paper_new_id": 105, "id": "j_8313d7d78cba293a79e1d714d857a4af", "title+abstract": "Fabrication and efficient photocatalytic degradation of methylene blue over CuO/BiVO4 composite under visible-light irradiation;Abstract CuO/BiVO 4 composite photocatalysts were prepared by solution combustion synthesis method and impregnation technique. X-ray diffraction, X-ray photoelectron spectroscopy, field-emission scan electron microscopy and UV¡§Cvis diffusion reflectance spectra were used to identify the physical properties and photophysical properties of CuO/BiVO 4 composite photocatalysts. The photocatalysts exhibit the enhanced photocatalytic properties for degradation of methylene blue under visible-light ( |? ?>?420?nm). The mechanism of improved photocatalytic activity is also discussed.", "title+abstract_embedding_0": -0.4871077, "title+abstract_embedding_1": 1.7857896, "title+abstract_embedding_2": -0.023201764, "title+abstract_embedding_3": -0.33812165, "title+abstract_embedding_4": -0.29073453, "title+abstract_embedding_5": -0.52627397, "title+abstract_embedding_6": -0.09837741, "title+abstract_embedding_7": 0.13212061, "title+abstract_embedding_8": 0.38774037, "title+abstract_embedding_9": -0.29044288, "title+abstract_embedding_10": -0.006995134, "title+abstract_embedding_11": 0.26866338, "title+abstract_embedding_12": -0.18413675, "title+abstract_embedding_13": -0.2816505, "title+abstract_embedding_14": -0.04232377, "title+abstract_embedding_15": 0.054195546, "title+abstract_embedding_16": 0.3047279, "title+abstract_embedding_17": -0.38274476, "title+abstract_embedding_18": -0.08778603, "title+abstract_embedding_19": 0.1550233, "title+abstract_embedding_20": 0.5262974, 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"title+abstract_embedding_89": 0.100799896, "title+abstract_embedding_90": -0.06535708, "title+abstract_embedding_91": -0.0991335, "title+abstract_embedding_92": 0.054121405, "title+abstract_embedding_93": -0.18000749, "title+abstract_embedding_94": 0.1034828, "title+abstract_embedding_95": -0.04067982, "title+abstract_embedding_96": -0.022689633, "title+abstract_embedding_97": -0.014631625, "title+abstract_embedding_98": 0.22605985, "title+abstract_embedding_99": 0.02301728, "title+abstract_embedding_100": 0.007166401, "title+abstract_embedding_101": -0.038448077, "title+abstract_embedding_102": 0.009569604, "title+abstract_embedding_103": 0.029402778, "title+abstract_embedding_104": 0.050757736, "title+abstract_embedding_105": -0.01611571, "title+abstract_embedding_106": 0.08893604, "title+abstract_embedding_107": 0.035510667, "title+abstract_embedding_108": 0.060921997, "title+abstract_embedding_109": -0.048151806, "title+abstract_embedding_110": -0.04774688, "title+abstract_embedding_111": 0.006973714, "title+abstract_embedding_112": -0.051046863, "title+abstract_embedding_113": 0.014475279, "title+abstract_embedding_114": -0.048955165, "title+abstract_embedding_115": 0.09560213, "title+abstract_embedding_116": 0.12269437, "title+abstract_embedding_117": 0.03702984, "title+abstract_embedding_118": -0.005657467, "title+abstract_embedding_119": -0.20088871, "title+abstract_embedding_120": 0.05230893, "title+abstract_embedding_121": -0.100451626, "title+abstract_embedding_122": -0.056582183, "title+abstract_embedding_123": -0.08038345, "title+abstract_embedding_124": 0.049052887, "title+abstract_embedding_125": -0.09213304, "title+abstract_embedding_126": -0.016551618, "title+abstract_embedding_127": -0.15043184, "label": 1, "label-multi": "1" }, { "paper_new_id": 106, "id": "j_838803fd82563583e3391b651dcd32c1", "title+abstract": "Edge-Terminated MoS2\n Nanoassembled Electrocatalyst via In Situ Hybridization with 3D Carbon Network;Transition metal dichalcogenides, especially MoS2 , are considered as promising electrocatalysts for hydrogen evolution reaction (HER). Since the physicochemical properties of MoS2 and electrode morphology are highly sensitive factor for HER performance, designed synthesis is highly pursued. Here, an in situ method to prepare a 3D carbon/MoS2 hybrid catalyst, motivated by the graphene ribbon synthesis process, is reported. By rational design strategies, the hybrid electrocatalysts with cross-connected porous structure are obtained, and they show a high HER activity even comparable to the state-of-the-art MoS2 catalyst without appreciable activity loss in long-term operations. Based on various physicochemical techniques, it is demonstrated that the synthetic procedure can effectively guide the formation of active site and 3D structure with a distinctive feature; increased exposure of active sites by decreased domain size and intrinsically high activity through controlling the number of stacking layers. Moreover, the importance of structural properties of the MoS2 -based catalysts is verified by controlled experiments, validating the effectiveness of the designed synthesis approach.", "title+abstract_embedding_0": -0.576173, "title+abstract_embedding_1": -0.7052293, "title+abstract_embedding_2": -0.2227703, "title+abstract_embedding_3": -0.21640182, "title+abstract_embedding_4": 0.19018584, "title+abstract_embedding_5": 0.2128931, "title+abstract_embedding_6": -0.25445607, "title+abstract_embedding_7": -0.50986993, "title+abstract_embedding_8": 0.105936624, "title+abstract_embedding_9": 0.8536334, "title+abstract_embedding_10": 0.17903265, "title+abstract_embedding_11": -0.030578716, "title+abstract_embedding_12": 0.14691022, "title+abstract_embedding_13": 0.1313527, "title+abstract_embedding_14": 0.13159627, "title+abstract_embedding_15": -0.1686936, "title+abstract_embedding_16": -0.14210601, "title+abstract_embedding_17": -0.51621777, "title+abstract_embedding_18": -0.3618282, 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"title+abstract_embedding_109": 0.071378306, "title+abstract_embedding_110": -0.14808857, "title+abstract_embedding_111": -0.060150422, "title+abstract_embedding_112": 0.17760463, "title+abstract_embedding_113": -0.038177952, "title+abstract_embedding_114": -0.117560744, "title+abstract_embedding_115": -0.025910847, "title+abstract_embedding_116": -0.034910306, "title+abstract_embedding_117": -0.047817715, "title+abstract_embedding_118": -0.12550825, "title+abstract_embedding_119": -0.13182938, "title+abstract_embedding_120": -0.014046544, "title+abstract_embedding_121": -0.02399209, "title+abstract_embedding_122": 0.16469982, "title+abstract_embedding_123": 0.068031855, "title+abstract_embedding_124": -0.16511348, "title+abstract_embedding_125": 0.024085637, "title+abstract_embedding_126": -0.013145844, "title+abstract_embedding_127": 0.04119069, "label": 3, "label-multi": "1;15;2;3" }, { "paper_new_id": 107, "id": "j_84c6e19cb5d2be4dd2cb1ea268463e7a", "title+abstract": "Optimization of parameters on photocatalytic degradation of chloramphenicol using TiO2 as photocatalyist by response surface methodology;The experimental design methodology was applied for modeling and optimizing the operation parameters on photocatalytic degradation of chloramphenicol (CAP) using TiO_2 as photocatalyst in a photoreactor. Three experimental parameters (including pH, TiO_2 concentration and CAP initial concentration) were adopted to obtain the preliminary information. The multivariate experimental design was employed to establish a quadratic model as a functional relationship between the degradation rate of CAP and three experimental parameters. The interaction effects and optimal parameters were obtained by using Design Expert software. The optimal values of the operation parameters under the related constraint conditions were found at pH 6.4, TiO_2 concentration of 0.94 g/L and CAP initial concentration of 19.97 mg/L, respectively. The degradation rate of CAP approached 85.97% under optimal conditions. The regression analysis with R2 value of 0.9519 had a good agreement between the experimental results and the predictive values. In addition, pH and TiO2 concentration had a significant influence on the degradation rate of CAP", "title+abstract_embedding_0": 0.06533754, "title+abstract_embedding_1": 0.701553, "title+abstract_embedding_2": 1.257773, "title+abstract_embedding_3": 1.201257, "title+abstract_embedding_4": 0.40233618, "title+abstract_embedding_5": -0.1023525, "title+abstract_embedding_6": -0.067362696, "title+abstract_embedding_7": -0.39582866, "title+abstract_embedding_8": 0.088512965, "title+abstract_embedding_9": 0.41834772, "title+abstract_embedding_10": -0.09874474, "title+abstract_embedding_11": -0.12681001, "title+abstract_embedding_12": 0.000361383, "title+abstract_embedding_13": -0.1645295, "title+abstract_embedding_14": -0.013330638, "title+abstract_embedding_15": 0.121488504, "title+abstract_embedding_16": 0.17159018, "title+abstract_embedding_17": -0.462134, "title+abstract_embedding_18": -0.18531013, "title+abstract_embedding_19": -0.21945065, "title+abstract_embedding_20": 0.538518, 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"title+abstract_embedding_112": 0.12728536, "title+abstract_embedding_113": 0.09792318, "title+abstract_embedding_114": 0.016133308, "title+abstract_embedding_115": -0.13535005, "title+abstract_embedding_116": 0.14684165, "title+abstract_embedding_117": 0.11763285, "title+abstract_embedding_118": -0.049314905, "title+abstract_embedding_119": 0.014926316, "title+abstract_embedding_120": -0.007585198, "title+abstract_embedding_121": 0.05034584, "title+abstract_embedding_122": 0.19376847, "title+abstract_embedding_123": -0.09309788, "title+abstract_embedding_124": -0.06986868, "title+abstract_embedding_125": 0.036935125, "title+abstract_embedding_126": -0.056132957, "title+abstract_embedding_127": -0.000674069, "label": 16, "label-multi": "16" }, { "paper_new_id": 108, "id": "j_851f0f718a7a36f04213aa4df144c53a", "title+abstract": "Photocatalytic degradation of microcystin-LR using TiO2 nanotubes under irradiation with UV and natural sunlight;In order to investigate the catalytic performance of anodic TiO2 nanotubes and their practical application in the treatment of refractory microcystins (MCs) in natural-water samples, TiO2 nanotubes of diameter of 50-80 nm were fabricated by anodization in C2H2O4 center dot 2H(2)O containing NH4F. Under irradiation with natural sunlight, MC-LR was totally degraded after 1 d using the anodic TiO2 nanotubes. In contrast, the removal efficiency without TiO2 nanotubes was as low as 47.7% within 20 d. In addition, a mixture of anatase and rutile TiO2 gave higher photocatalytic activity than the single phase did. The pH also influenced the adsorption capacity of the TiO2 nanotubes. The order of MC-LR degradation efficiencies at different pH values was 3.5 > 8.0 > 10.0. After five repeated experiments on the degradation of MC-LR for 7 h, the degradation efficiency was still stable.", "title+abstract_embedding_0": 0.2826811, "title+abstract_embedding_1": 0.64926326, "title+abstract_embedding_2": 0.0936248, "title+abstract_embedding_3": 0.986754, "title+abstract_embedding_4": 0.33793133, "title+abstract_embedding_5": -0.10979426, "title+abstract_embedding_6": -0.20840505, "title+abstract_embedding_7": -0.46139583, "title+abstract_embedding_8": -0.1439933, "title+abstract_embedding_9": 0.14043888, "title+abstract_embedding_10": -0.4614604, "title+abstract_embedding_11": -0.3560431, "title+abstract_embedding_12": -0.10741776, "title+abstract_embedding_13": 0.1549407, "title+abstract_embedding_14": -0.06296314, "title+abstract_embedding_15": -0.52905226, "title+abstract_embedding_16": 0.35243446, "title+abstract_embedding_17": -0.07171969, "title+abstract_embedding_18": 0.31762666, "title+abstract_embedding_19": 0.13681594, "title+abstract_embedding_20": 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"title+abstract_embedding_66": -0.17424965, "title+abstract_embedding_67": 0.06512365, "title+abstract_embedding_68": 0.2591167, "title+abstract_embedding_69": 0.05595629, "title+abstract_embedding_70": 0.056161482, "title+abstract_embedding_71": 0.15397497, "title+abstract_embedding_72": -0.28373295, "title+abstract_embedding_73": 0.20658125, "title+abstract_embedding_74": -0.002386995, "title+abstract_embedding_75": -0.041391127, "title+abstract_embedding_76": 0.04156387, "title+abstract_embedding_77": 0.009090573, "title+abstract_embedding_78": -0.064786986, "title+abstract_embedding_79": -0.08412987, "title+abstract_embedding_80": -0.045697566, "title+abstract_embedding_81": -0.15673321, "title+abstract_embedding_82": 0.06611237, "title+abstract_embedding_83": 0.003586347, "title+abstract_embedding_84": -0.11023946, "title+abstract_embedding_85": 0.048720524, "title+abstract_embedding_86": -0.007958606, "title+abstract_embedding_87": -0.10699884, "title+abstract_embedding_88": 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"title+abstract_embedding_111": -0.071724236, "title+abstract_embedding_112": -0.0885755, "title+abstract_embedding_113": -0.009291843, "title+abstract_embedding_114": 0.105047226, "title+abstract_embedding_115": -0.057587363, "title+abstract_embedding_116": 0.049021713, "title+abstract_embedding_117": 0.14659128, "title+abstract_embedding_118": -0.031431865, "title+abstract_embedding_119": 0.124771, "title+abstract_embedding_120": -0.14292365, "title+abstract_embedding_121": 0.046653282, "title+abstract_embedding_122": 0.0594123, "title+abstract_embedding_123": -0.14263426, "title+abstract_embedding_124": 0.066855505, "title+abstract_embedding_125": 0.21001208, "title+abstract_embedding_126": 0.018498473, "title+abstract_embedding_127": 0.008574888, "label": 106, "label-multi": NaN }, { "paper_new_id": 109, "id": "j_85df1642b63ba00987b64efbec3def20", "title+abstract": "Probing the photolytica??photocatalytic degradation mechanism of DEET in the presence of natural or synthetic humic macromolecules using molecular-scavenging techniques and EPR spectroscopy;Abstract The present work provides for the first time a detailed investigation of the photolytic and photocatalytic degradation mechanisms of DEET in the presence of different types of dissolved organic matter (DOM) e.g., a lignite HA (LHA) mainly of aliphatic character, a synthetic humic acid like polycondensate (HALP) with aromatic-ring rich properties and a soil fulvic acid (FA). The data are based on catalytic, molecular-scavenging and electron paramagnetic resonance (EPR) experiments. Photodegradation rates were significantly increased in the presence of different humic and fulvic acids and were highly dependent upon DOM composition, whereas they reached a threshold at approximately 1.0?mg?L?1 of DOM. Scavenging experiments indicated that excited state DOM* plays a key role in the photochemical transformation in the presence of the studied humic and fulvic acids. FA and HALP showed an increasing trend in the photocatalytic degradation kinetics, while retardation was observed in the presence of LHA. EPR spin-trapping measurements in the presence of TiO2, showed that DOM type affect the generation of HO and the hydroxy-DEET-radicals which are formed in the initial steps of photodegradation. Fulvic acid was found to have the less significant effect on HO formation, while it contributed significantly to the photocatalytic degradation through a sensitization/charge injection mechanism with subsequent formation of O2 ? and 1O2.", "title+abstract_embedding_0": 0.6581149, "title+abstract_embedding_1": 0.43615723, "title+abstract_embedding_2": 1.0346223, "title+abstract_embedding_3": -0.040346026, "title+abstract_embedding_4": -0.6681558, "title+abstract_embedding_5": -0.2586621, "title+abstract_embedding_6": -0.2276831, "title+abstract_embedding_7": 0.051768605, "title+abstract_embedding_8": 0.1575326, "title+abstract_embedding_9": -0.035669386, "title+abstract_embedding_10": -0.09931701, "title+abstract_embedding_11": 0.25884044, "title+abstract_embedding_12": -0.06527752, "title+abstract_embedding_13": 0.095303364, "title+abstract_embedding_14": 0.17364761, "title+abstract_embedding_15": 0.09138211, "title+abstract_embedding_16": 0.3517027, "title+abstract_embedding_17": 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"title+abstract_embedding_107": 0.15247875, "title+abstract_embedding_108": -0.045005046, "title+abstract_embedding_109": -0.083179206, "title+abstract_embedding_110": 0.057747453, "title+abstract_embedding_111": -0.02347027, "title+abstract_embedding_112": -0.02110751, "title+abstract_embedding_113": 0.13394435, "title+abstract_embedding_114": 0.059344754, "title+abstract_embedding_115": 0.007791817, "title+abstract_embedding_116": 0.016811784, "title+abstract_embedding_117": 0.062490582, "title+abstract_embedding_118": 0.123217486, "title+abstract_embedding_119": 0.02355928, "title+abstract_embedding_120": 0.0800647, "title+abstract_embedding_121": -0.032098815, "title+abstract_embedding_122": -0.020637423, "title+abstract_embedding_123": 0.003055349, "title+abstract_embedding_124": 0.002324671, "title+abstract_embedding_125": 0.002389014, "title+abstract_embedding_126": -0.09657087, "title+abstract_embedding_127": 0.06993719, "label": 106, "label-multi": NaN }, { "paper_new_id": 110, "id": "j_866b19d6c3a8bc78d05c615e1be5394c", "title+abstract": "MoS2/Cu2O nanohybrid as a highly efficient catalyst for the photoelectrocatalytic hydrogen generation;Abstract To improve the low photocatalytic efficiency of Cu2O caused by the serious photo-generated electron-hole recombination, in this work, MoS2 is proposed to combine with Cu2O to form a nanohybrid as a photo-electrocatalytic catalyst for hydrogen generation. It is found that the optimized hybrid catalyst of 50M-C exhibits the best performance with a current density of 3700?|¨¬A cm?2 at ?1.2?V (vs SCE), which is approximately 18-fold and 8-fold higher than those of single MoS2 (200?|¨¬A?cm?2) and Cu2O (450?|¨¬A?cm?2), respectively. Moreover, the enhancement mechanism is also discussed, and a synergistic effect between MoS2 and Cu2O is verified, which can reduce the charge transfer resistance and accelerate the separation of photo-generated electrons and holes.", "title+abstract_embedding_0": -0.40053242, "title+abstract_embedding_1": 0.43217212, "title+abstract_embedding_2": -0.08105114, "title+abstract_embedding_3": -0.52345514, "title+abstract_embedding_4": 0.37048012, "title+abstract_embedding_5": 0.2189515, "title+abstract_embedding_6": 0.671325, "title+abstract_embedding_7": -0.77047944, "title+abstract_embedding_8": 0.08700619, "title+abstract_embedding_9": 0.1783084, "title+abstract_embedding_10": 0.076953605, "title+abstract_embedding_11": 0.06126736, "title+abstract_embedding_12": -0.65747297, "title+abstract_embedding_13": 0.4240212, "title+abstract_embedding_14": -0.5363529, "title+abstract_embedding_15": -0.16516623, "title+abstract_embedding_16": -0.023733556, "title+abstract_embedding_17": 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"title+abstract_embedding_63": -0.018532045, "title+abstract_embedding_64": -0.020391434, "title+abstract_embedding_65": 0.06559898, "title+abstract_embedding_66": 0.15051806, "title+abstract_embedding_67": 0.09817135, "title+abstract_embedding_68": -0.0671869, "title+abstract_embedding_69": -0.13320738, "title+abstract_embedding_70": -0.096746735, "title+abstract_embedding_71": 0.13676466, "title+abstract_embedding_72": -0.060831606, "title+abstract_embedding_73": 0.031899553, "title+abstract_embedding_74": -0.15509096, "title+abstract_embedding_75": 0.06839231, "title+abstract_embedding_76": -0.023392648, "title+abstract_embedding_77": 0.008406565, "title+abstract_embedding_78": -0.06334429, "title+abstract_embedding_79": -0.0444576, "title+abstract_embedding_80": 0.014495295, "title+abstract_embedding_81": 0.010424387, "title+abstract_embedding_82": 0.12917271, "title+abstract_embedding_83": -0.09103776, "title+abstract_embedding_84": 0.04303047, "title+abstract_embedding_85": 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"title+abstract_embedding_108": -0.057868462, "title+abstract_embedding_109": 0.004938975, "title+abstract_embedding_110": 0.057225645, "title+abstract_embedding_111": 0.071238175, "title+abstract_embedding_112": 0.07149416, "title+abstract_embedding_113": 0.03890474, "title+abstract_embedding_114": -0.061421283, "title+abstract_embedding_115": 0.036066703, "title+abstract_embedding_116": -0.15024815, "title+abstract_embedding_117": 0.081591934, "title+abstract_embedding_118": -0.065189384, "title+abstract_embedding_119": 0.026944276, "title+abstract_embedding_120": 0.052580167, "title+abstract_embedding_121": -0.02331253, "title+abstract_embedding_122": 0.000936747, "title+abstract_embedding_123": 0.07292258, "title+abstract_embedding_124": 0.115086585, "title+abstract_embedding_125": 0.13809298, "title+abstract_embedding_126": 0.06288624, "title+abstract_embedding_127": -0.049166963, "label": 1, "label-multi": "1;2" }, { "paper_new_id": 111, "id": "j_87a49c6a5a4d15a5768cc94e8d8af841", "title+abstract": "Facile self-assembly synthesis of ?3-Fe2O3 /graphene oxide for enhanced photo-Fenton reaction;A novel self-assembly method was developed to prepare a |?-Fe2O3/graphene oxide (GO) heterogeneous catalyst that showed excellent synergy between photocatalysis and Fenton-like reactions. The |?-Fe2O3/GO catalyst prepared on the iron plates demonstrated efficient and reproducible catalytic activities for water treatment. It takes only 80?min to degrade 50?mg?L-1 methylene (MB) completely, which is the main non-biodegradable dye in wastewater from the textile industry. The heterogeneous catalyst is stable over a wide range of pH (from 2.0 to 10.2) for MB degradation, and can be easily extracted from solution and repeatedly used with little loss of catalytic activity. The high activity and stability of the catalyst system can be attributed to charge separation between |?-Fe2O3 and GO, which could accelerate Fenton-like process and photocatalysis. In addition, the dominant reactive oxidant species responsible for the MB degradation, including the hydroxyl radicals (?OH) and holes (h+), were trapped on the surface of the |?-Fe2O3/GO composite, as proved by a free-radical quenching experiment. The |?-Fe2O3/GO heterogeneous catalyst could potentially provide a solution for removal of non-biodegradable dyes from wastewater in the textile industry.", "title+abstract_embedding_0": 0.3688959, "title+abstract_embedding_1": -0.03708902, "title+abstract_embedding_2": 0.21639718, "title+abstract_embedding_3": -0.52420247, "title+abstract_embedding_4": 0.614518, "title+abstract_embedding_5": -0.20265192, "title+abstract_embedding_6": -0.61236477, "title+abstract_embedding_7": 0.07126534, "title+abstract_embedding_8": 0.053683985, "title+abstract_embedding_9": 0.40335715, "title+abstract_embedding_10": -0.18656392, "title+abstract_embedding_11": 0.1950765, "title+abstract_embedding_12": -0.2657158, "title+abstract_embedding_13": -0.30911648, "title+abstract_embedding_14": 0.2931116, "title+abstract_embedding_15": -0.08403958, "title+abstract_embedding_16": -0.012421459, "title+abstract_embedding_17": 0.089904904, "title+abstract_embedding_18": 0.22346403, "title+abstract_embedding_19": 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"title+abstract_embedding_87": 0.021817375, "title+abstract_embedding_88": -0.07342419, "title+abstract_embedding_89": -0.027112983, "title+abstract_embedding_90": 0.06126885, "title+abstract_embedding_91": 0.107651755, "title+abstract_embedding_92": 0.03763677, "title+abstract_embedding_93": -0.042542405, "title+abstract_embedding_94": -0.15858932, "title+abstract_embedding_95": -0.13022864, "title+abstract_embedding_96": 0.01434052, "title+abstract_embedding_97": -0.005386594, "title+abstract_embedding_98": -0.010537688, "title+abstract_embedding_99": 0.11649322, "title+abstract_embedding_100": -0.04728295, "title+abstract_embedding_101": -0.03774335, "title+abstract_embedding_102": 0.06953946, "title+abstract_embedding_103": -0.061508663, "title+abstract_embedding_104": -0.16166404, "title+abstract_embedding_105": -0.10296823, "title+abstract_embedding_106": -0.02780141, "title+abstract_embedding_107": 0.004066437, "title+abstract_embedding_108": -0.23864265, "title+abstract_embedding_109": 0.0192253, "title+abstract_embedding_110": 0.014822751, "title+abstract_embedding_111": 0.14420971, "title+abstract_embedding_112": -0.1442502, "title+abstract_embedding_113": -0.14458443, "title+abstract_embedding_114": 0.04704286, "title+abstract_embedding_115": 0.014654473, "title+abstract_embedding_116": 0.038577415, "title+abstract_embedding_117": -0.07677694, "title+abstract_embedding_118": -0.03004992, "title+abstract_embedding_119": 0.22178386, "title+abstract_embedding_120": -0.015318153, "title+abstract_embedding_121": 0.12697667, "title+abstract_embedding_122": -0.012014747, "title+abstract_embedding_123": 0.000517741, "title+abstract_embedding_124": -0.021638162, "title+abstract_embedding_125": 0.002233192, "title+abstract_embedding_126": 0.012871139, "title+abstract_embedding_127": -0.026128829, "label": 16, "label-multi": "16" }, { "paper_new_id": 112, "id": "j_893aa7f94cf1c6ef2768a3d7042cfd1b", "title+abstract": "A platinised TiO2 film with both photocatalytic and non-photocatalytic activities towards the oxidation of formic acid;Abstract A platinised TiO 2 /ITO film, Pt-TiO 2 /ITO, was prepared by a dip-coating and subsequent photodeposition procedure. Compared with bare TiO 2 /ITO film, Pt-TiO 2 /ITO film not only possesses a relative high photocatalytic activity but also shows a rather non-photocatalytic activity towards HCOOH degradation at room temperature and atmosphere pressure. The non-photocatalytic effect of platinised TiO 2 was partly responsible for degradation of formic acid in the photocatalytic process. The non-photocatalytic activity of Pt-TiO 2 /ITO film is very dependent on its preparation method.", "title+abstract_embedding_0": -0.11205995, "title+abstract_embedding_1": 1.5776976, "title+abstract_embedding_2": -0.33933058, "title+abstract_embedding_3": 0.82554317, "title+abstract_embedding_4": 0.8948383, "title+abstract_embedding_5": 0.43513066, "title+abstract_embedding_6": -0.006376445, "title+abstract_embedding_7": 0.10273476, "title+abstract_embedding_8": -0.19051744, "title+abstract_embedding_9": 0.071397156, "title+abstract_embedding_10": 0.47202545, "title+abstract_embedding_11": -0.08633157, "title+abstract_embedding_12": 0.41803396, "title+abstract_embedding_13": -0.20045301, "title+abstract_embedding_14": -0.32075453, "title+abstract_embedding_15": 0.07978602, "title+abstract_embedding_16": -0.27113461, "title+abstract_embedding_17": -0.3471265, "title+abstract_embedding_18": 0.002563126, "title+abstract_embedding_19": -0.20884962, "title+abstract_embedding_20": 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Films;2¨¦¨®???3??¡è1a3¨¢?y¨º?(PLD)¨ª??¨º¨ªa?¨®¨¦¨²3¡è¨¢?¡Ã¨ª???-¡Ã¨®??????¦Ã?6%(?-¡Ã¨®¡Ã¨¨)Cr2??¨®¦Ã??eo¨¬¨º¡¥?¨¤TiO_2(110)¦Ã£¤?¡ì¡Ã??¡è,2¨¦¨®?¨¦¡§?¨¨?¨ª¦Ã¨¤???¡é?¦Ã(STM)?¡é¨¦¡§?¨¨?¨ª¦Ã¨¤?¡Ã(STS)?¡éX¨¦???1a¦Ã?¡Ã¨®?¨¹?¡Ã(XPS)o¨ª¡Ã?¨ªa1a¦Ã?¡Ã¨®?¨¹?¡Ã(UPS)??????DD¨¢?¡Ã¨ª?¡Ã.?¨¢1?¡Ã¨ª?¡Ã:Cr2??¨®??TiO_2(110)-(1?¨¢1)¡Ã¨ª??¦Ã?D??2??¨®D?¡Ã??¨®¡ã?¨¬,¦Ã?¨º?¨¬¨¢??¨¢?2??¨®¡Ã??¡è?¨²?o???1¦Ã?¦Ã?¦Ã?D?;Cr¨®??¡ì??O?¨¹o???3¨º??+3??¨¬?,¨®¨¦¡ä??¨²TiO_2¦Ã???¡ä??£¤¨¦?¡¤?~0.4eV¡ä|¨°y¨¨??¨®?¨º?¨¹??.¡Ã?¨ªa-?¨¦??1a?¨¹¨º??¡Ã??¨º?¡Ã??¡è¦Ã?1a?¨¹¨º??¨¹¨¢|¡Ã?¨¤??1¦Ã?~650nm,¡ä|¨®¨²?¨¦??1a¡¤??¡ì.?¨¨?¨²STM¨°?¦Ã£¤???¡Ã¡ä?¡¤?¡Ã¨®¦Ã?1a?a¡¤¡ä¨®|?¨¬2a¨¢?¡Ã??¡è¦Ã?1a¡ä??¡¥??D?.??1?2¨¬¦Ã?¡Ã?¨ªa1a??¨¦????¡Ã¡ä?¡¤?¡Ã¨®¦Ã?¨ª??a¡¤¡ä¨®|,?¨²?¨¦??1a??¨¦???(|?>430nm)?¡Ã¡ä?¡¤?¡Ã¨®??¨®D¡¤¡é¨¦¨²¡¤¡ä¨®|,¡Ã¨ª?¡Ã¦Ã£¤?¨¤¦Ã?Cr2??¨®?¨¦?¨¹2?¡Ã?¨°?¨¬¨¢??TiO_2?¨²?¨¦??1a??¦Ã?¡ä??¡¥??D?.", "title+abstract_embedding_0": 0.5060102, "title+abstract_embedding_1": 0.23350096, "title+abstract_embedding_2": 1.0435336, "title+abstract_embedding_3": 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"title+abstract_embedding_118": -0.11714079, "title+abstract_embedding_119": -0.06510639, "title+abstract_embedding_120": 0.49295262, "title+abstract_embedding_121": 0.14448369, "title+abstract_embedding_122": -0.1992664, "title+abstract_embedding_123": -0.20951624, "title+abstract_embedding_124": -0.45960593, "title+abstract_embedding_125": -0.14421329, "title+abstract_embedding_126": -0.11488737, "title+abstract_embedding_127": -0.19466797, "label": 3, "label-multi": "3" }, { "paper_new_id": 114, "id": "j_8b001cfc3461ada7fc08ba42ec58f8de", "title+abstract": "Graphene Supported Rhodium Nanoparticles for Enhanced Electrocatalytic Hydrogen Evolution Reaction;A PABA grafted Tix aerogel has both porous and semiconductive properties. The porosity, band gap, conductivity and even PL intensity of the aerogel are adjustable. The aerogel exhibited efficient photocatalytic performance in reduction of CO2.
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"title+abstract_embedding_113": -0.10060966, "title+abstract_embedding_114": 0.0801893, "title+abstract_embedding_115": -0.1334317, "title+abstract_embedding_116": 0.0426858, "title+abstract_embedding_117": -0.093023226, "title+abstract_embedding_118": -0.10239621, "title+abstract_embedding_119": 0.05633014, "title+abstract_embedding_120": 0.19708401, "title+abstract_embedding_121": 0.1764988, "title+abstract_embedding_122": -0.1047166, "title+abstract_embedding_123": 0.08610316, "title+abstract_embedding_124": -0.13955379, "title+abstract_embedding_125": 0.01747673, "title+abstract_embedding_126": 0.082748964, "title+abstract_embedding_127": -0.115133226, "label": 3, "label-multi": "3" }, { "paper_new_id": 149, "id": "j_c16cb5d2b9405335a7a72b772c4eaf2b", "title+abstract": "Phase Transition of Two-Dimensional ?2-Ga2O3 Nanosheets from Ultrathin ?3-Ga2O3 Nanosheets and Their Photocatalytic Hydrogen Evolution Activities;Monoclinic beta-Ga2O3 nanosheets hold great potential applications in electronic, optical, and photocatalytic fields. In this study, two-dimensional beta-Ga2O3 nanosheets were successfully fabricated through a simple crystalline phase transition from the as prepared ultrathin gamma-Ga2O3 nanosheets. The photocatalytic hydrogen evolution reaction under UV light irradiation was achieved on the two kinds of photocatalysts.However, beta-Ga2O3 with a higher crystallinity' shows a lower photocatalytic activity in comparison with gamma-Ga2O3. The average apparent quantum yield is calculated to be 0.29% for beta-Ga2O3 nanosheets and 1.82% for gamma-Ga2O3 . More efficient separation and transfer rates of photogenerated carriers and larger specific areas were found in gamma-Ga2O3. On the basis of the analysis of the structures of gamma-Ga2O and beta-Ga2O3, it is proposed that the disordered or defective structure contributes to the improvement of photocatalytic activity to some extent. Therefore, it is significant to develop the photocatalyst defects at the same time.", "title+abstract_embedding_0": 0.66724205, "title+abstract_embedding_1": 0.799858, "title+abstract_embedding_2": -0.3753167, "title+abstract_embedding_3": -0.45259595, "title+abstract_embedding_4": 0.06843984, "title+abstract_embedding_5": 0.34829402, "title+abstract_embedding_6": 0.3644999, "title+abstract_embedding_7": -0.22774914, "title+abstract_embedding_8": -0.41290012, "title+abstract_embedding_9": 0.33914262, "title+abstract_embedding_10": 0.52667344, "title+abstract_embedding_11": 0.10216394, "title+abstract_embedding_12": 0.20038363, "title+abstract_embedding_13": -0.14601392, "title+abstract_embedding_14": 0.063206285, "title+abstract_embedding_15": -0.50835145, "title+abstract_embedding_16": 0.30261868, "title+abstract_embedding_17": -0.1913411, "title+abstract_embedding_18": -0.053442836, "title+abstract_embedding_19": -0.11126095, "title+abstract_embedding_20": 0.1799364, 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"title+abstract_embedding_111": 0.087708436, "title+abstract_embedding_112": 0.002695426, "title+abstract_embedding_113": -0.020382628, "title+abstract_embedding_114": 0.1266509, "title+abstract_embedding_115": 0.080694795, "title+abstract_embedding_116": 0.058803998, "title+abstract_embedding_117": -0.039517075, "title+abstract_embedding_118": -0.040160585, "title+abstract_embedding_119": 0.117519885, "title+abstract_embedding_120": -0.06854886, "title+abstract_embedding_121": -0.017835202, "title+abstract_embedding_122": 0.019130558, "title+abstract_embedding_123": 0.048088275, "title+abstract_embedding_124": -0.002419718, "title+abstract_embedding_125": -0.028800547, "title+abstract_embedding_126": -0.06441054, "title+abstract_embedding_127": 0.002854005, "label": 3, "label-multi": "3" }, { "paper_new_id": 150, "id": "j_c2ce8a4e46a3f3c09e8c3b6e29fe2779", "title+abstract": "Effect of Synthesis Conditions of Nitrogen and Platinum Co-Doped Titania Films on the Photocatalytic Performance under Simulated Solar Light;The Ni2P cocatalyst can boost hydrogen generation over TiO2, CdS, and C3N4 photocatalysts, which demonstrates its good catalytic property and general applicability.
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"title+abstract_embedding_114": -0.26331806, "title+abstract_embedding_115": -0.03227354, "title+abstract_embedding_116": -0.06308286, "title+abstract_embedding_117": 0.2606011, "title+abstract_embedding_118": -0.14947538, "title+abstract_embedding_119": -0.12167008, "title+abstract_embedding_120": -0.017361045, "title+abstract_embedding_121": -0.041503765, "title+abstract_embedding_122": -0.21866557, "title+abstract_embedding_123": 0.030981943, "title+abstract_embedding_124": -0.12063164, "title+abstract_embedding_125": -0.1534597, "title+abstract_embedding_126": 0.02728178, "title+abstract_embedding_127": 0.074174196, "label": 3, "label-multi": "3" }, { "paper_new_id": 170, "id": "j_dd24953c472ca2b6b5141a4eb1ee296f", "title+abstract": "Photonic Switching Porous Organic Polymers toward Reversible Control of Heterogeneous Photocatalysis;Sonogashira-Hagihara coupling reaction of photoswitchable dithienylethene (AEDTE) with metal-free 5,10,15,20-tetrakis(4-iodophenyl)porphyrin and its metal derivatives (MTIPP, M = H-2, Zn(II), Fe(II)) results in three porous organic polymers (POPS) including AEDTE-H2TIPP-POP, AEDTE-ZnTIPP-POP, and AEDTE-FeTIPP-POP. The morphology, components, and structures of newly obtained POPs have been examined by a range of spectroscopic and microscopic techniques including infrared spectroscopy (IR), solid-state UV-vis diffuse reflectance spectroscopy, thermogravimetric analysis (TGA), powder X-ray diffraction, scanning electron microscopy, and transmission electron microscopy. The porous structures have been estimated by nitrogen and carbon dioxide sorption isotherms at 77 and 196 K, respectively. The open-AEDTE-H-2 TIPP-POP with AEDTE in an open form was revealed to be an effective and stable heterogeneous photocatalyst for visible light-driven oxidation of N-methylpyridinium salts possibly because of its relatively large specific surface area. In particular, a proof-of-concept of photoswitchable POP photocatalysts has been established using different light irradiation upon open-AEDTE-H2TIPP-POP to control its heterogeneous photocatalytic behaviors because of the adjustment over the electron transfer process and porous structures through photoisomerization of AEDTE. The present result highlights the bright perspective of photoswitching POPs in the field of materials chemistry and catalysis community.", "title+abstract_embedding_0": 0.6601943, "title+abstract_embedding_1": -0.006665826, "title+abstract_embedding_2": 0.21747857, "title+abstract_embedding_3": -0.44244838, "title+abstract_embedding_4": -0.6762326, "title+abstract_embedding_5": 0.32861814, "title+abstract_embedding_6": -0.5042764, "title+abstract_embedding_7": 0.6064801, "title+abstract_embedding_8": -0.4627909, "title+abstract_embedding_9": -0.14562315, "title+abstract_embedding_10": 0.044692904, "title+abstract_embedding_11": -0.19452004, "title+abstract_embedding_12": 0.05543658, "title+abstract_embedding_13": -0.19199595, "title+abstract_embedding_14": 0.5105115, "title+abstract_embedding_15": 0.15343468, "title+abstract_embedding_16": -0.30335164, "title+abstract_embedding_17": -0.3194939, "title+abstract_embedding_18": -0.20126912, "title+abstract_embedding_19": 0.008097418, 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"title+abstract_embedding_110": 0.1801492, "title+abstract_embedding_111": 0.004849102, "title+abstract_embedding_112": 0.07869676, "title+abstract_embedding_113": -0.119955555, "title+abstract_embedding_114": -0.035655484, "title+abstract_embedding_115": 0.16712873, "title+abstract_embedding_116": 0.04884971, "title+abstract_embedding_117": -0.011730447, "title+abstract_embedding_118": -0.078714624, "title+abstract_embedding_119": 0.022495855, "title+abstract_embedding_120": 0.06978582, "title+abstract_embedding_121": -0.06081432, "title+abstract_embedding_122": -0.052552044, "title+abstract_embedding_123": 0.09972536, "title+abstract_embedding_124": -0.032492436, "title+abstract_embedding_125": 0.022566222, "title+abstract_embedding_126": -0.12054018, "title+abstract_embedding_127": -0.048930615, "label": 1, "label-multi": "1;15" }, { "paper_new_id": 171, "id": "j_ddfb09cd6a571869f5add68d5eb1a2b9", "title+abstract": "A novel and highly efficient Ag and GO co-synthesized ZnO nano photocatalyst for methylene blue dye degradation under UV irradiation;Abstract Heterogeneous photocatalysis is an effective and promising treatment technology for the removal of organic dye compounds in textile wastewater. Hybrid nanostructured semiconductor materials have been extensively applied and received greater attention in the last few decades. In this study, nano structured zinc oxide (ZnO) was doped by silver (Ag) and graphene oxide (GO) nanoparticles to synthesize Ag/GO/ZnO using the sol¡§Cgel technique followed by the heat treatment method. The hexagonal wurtzite structure of ZnO as observed by SEM was changed to lump/flake shape after doping with Ag and GO onto the ZnO crystal surface. FTIR confirms the stretching vibration of broad O¡§CH groups with adsorbed H2O molecules. The broad absorption edge of Ag/GO/ZnO nanocomposite shifted to the visible-light region with the reduced band gap energy of 3.22?eV as compared to 3.34 for ZnO. The photocatalytic degradation of methylene blue (MB) dye (15 mgL?1) under 100?W UV irradiation was84.67%, 88.13%, and 97.53%, for ZnO, Ag/ZnO, and Ag/GO/ZnO nanocomposites, respectively, at the same dose of photocatalyst (0.300?g) and pH 11.0for3 h UV irradiation. The best fitted kinetic of photocatalytic studies were showed a pseudo-first-order reaction model and the respective rate constants were found to be 0.0129?min?1, 0.0149?min?1, and 0.5198?min?1, for ZnO, Ag/ZnO, and Ag/GO/ZnO nanocomposites, respectively. The enriched photodegradation activity of Ag/GO/ZnO nanocomposite indicates the potential of the nanocomposite for the treatment of organic pollutants from the textile wastewater.", "title+abstract_embedding_0": 1.2727247, "title+abstract_embedding_1": 0.24392045, "title+abstract_embedding_2": -0.5056853, "title+abstract_embedding_3": -0.097566366, "title+abstract_embedding_4": -0.061525643, "title+abstract_embedding_5": -1.27629, "title+abstract_embedding_6": -0.19377169, "title+abstract_embedding_7": 0.41477033, "title+abstract_embedding_8": 0.11492091, "title+abstract_embedding_9": 0.16761965, "title+abstract_embedding_10": -0.686126, "title+abstract_embedding_11": -0.06257208, "title+abstract_embedding_12": 0.42080295, "title+abstract_embedding_13": -0.16941068, "title+abstract_embedding_14": -0.060085207, "title+abstract_embedding_15": 0.08485279, "title+abstract_embedding_16": -0.05375123, "title+abstract_embedding_17": 0.001515791, "title+abstract_embedding_18": -0.0997625, 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"title+abstract_embedding_109": -0.01863426, "title+abstract_embedding_110": -0.010867536, "title+abstract_embedding_111": 0.012210406, "title+abstract_embedding_112": -0.053892955, "title+abstract_embedding_113": -0.092452675, "title+abstract_embedding_114": -0.106251016, "title+abstract_embedding_115": -0.11899481, "title+abstract_embedding_116": 0.081717186, "title+abstract_embedding_117": 0.007411331, "title+abstract_embedding_118": -0.039066836, "title+abstract_embedding_119": 0.037085596, "title+abstract_embedding_120": -0.071209185, "title+abstract_embedding_121": -0.08039763, "title+abstract_embedding_122": -0.03639239, "title+abstract_embedding_123": -0.008293264, "title+abstract_embedding_124": -0.0950812, "title+abstract_embedding_125": -0.032730922, "title+abstract_embedding_126": -0.074981555, "title+abstract_embedding_127": -0.04325719, "label": 106, "label-multi": NaN }, { "paper_new_id": 172, "id": "j_df6f1eadcff007e32759bfb0edeb1091", "title+abstract": "Simple fabrication of twist-like helix N,S-codoped titania photocatalyst with visible-light response;Visible-light responsible N,S-codoped titania photocatalyst was fabricated by simple hydrolysis of titania tetrachloride using ammonia in the presence of glacial acetic acid and ammonium sulfate. The N,S-codoped titania materials were fabricated by a template-free route and demonstrated twist-like helix morphology. The morphology and microstructure characteristics of N,S-codoped titania photocatalysts were characterized by means of the N-2 adsorption-desorption measurements, thermal gravimetric and differential thermal analysis (TG-DTA), transmission electron microscopy (TEM), scanning electron microscopy (SEM), X-ray photoelectron spectroscopy (XPS), Fourier transform infrared spectroscopy (FT-IR), UV-visible diffuse reflectance spectra (DRS) and X-ray powder diffraction (XRD). The unique morphology of N,S-codoped titania materials and mesoporous microstructure were maintained after a heat treatment at 723 K for 3 h, exhibiting significantly thermal stability. The photocatalytic activity was evaluated by degrading phenol in aqueous suspension under ultraviolet and visible light irradiation. The results obtained with these novel photocatalysts are compared with the behavior of the well-studied and widely used Degussa P25 TiO2 under the same conditions. The N,S-codoped Titania samples were more superior than P25 and the sample calcined under 723 K for 3 h shows the best photocatalytic activity, the higher activity of which could be attributed to its high surface area, large pore volume, well-crystallized anatase, red-shift in adsorption edge and strong absorbance of light with longer wavelength. (C) 2007 Elsevier B.V. All rights reserved.", "title+abstract_embedding_0": 1.1147271, "title+abstract_embedding_1": 0.48067635, "title+abstract_embedding_2": -0.035834998, "title+abstract_embedding_3": 0.012359202, "title+abstract_embedding_4": 0.4932626, "title+abstract_embedding_5": 0.5088081, "title+abstract_embedding_6": 0.041152686, "title+abstract_embedding_7": 0.43662292, "title+abstract_embedding_8": -0.116114594, "title+abstract_embedding_9": -0.11943662, "title+abstract_embedding_10": 0.095251545, "title+abstract_embedding_11": 0.11867459, "title+abstract_embedding_12": -0.03677234, "title+abstract_embedding_13": 0.046050996, "title+abstract_embedding_14": 0.32418278, "title+abstract_embedding_15": 0.26480308, "title+abstract_embedding_16": 0.13020164, "title+abstract_embedding_17": 0.28834715, "title+abstract_embedding_18": 0.051095054, "title+abstract_embedding_19": -0.16456816, "title+abstract_embedding_20": -0.08282088, "title+abstract_embedding_21": -0.072595656, 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"title+abstract_embedding_112": -0.14306135, "title+abstract_embedding_113": 0.07228172, "title+abstract_embedding_114": -0.01543045, "title+abstract_embedding_115": 0.1507414, "title+abstract_embedding_116": 0.04422216, "title+abstract_embedding_117": -0.017894343, "title+abstract_embedding_118": -0.119774185, "title+abstract_embedding_119": -0.008740568, "title+abstract_embedding_120": 0.008213839, "title+abstract_embedding_121": -0.029833024, "title+abstract_embedding_122": -0.038865715, "title+abstract_embedding_123": 0.11249743, "title+abstract_embedding_124": 0.000529915, "title+abstract_embedding_125": 0.037606, "title+abstract_embedding_126": -0.005699407, "title+abstract_embedding_127": 0.13273855, "label": 3, "label-multi": "0;3" }, { "paper_new_id": 173, "id": "j_e0de5c1f839f9935e174a6d52e118a7d", "title+abstract": "The effective strategies of preparing black F-TiIII-codoping TiO2 anchored on sepiolite for enhanced photodegradation;Abstract Composition and color tailoring is an effective strategy for improving the efficiency of photocatalysts. In this study, black F-TiIII-codoping TiO2 (BFTiO2) was successfully prepared and anchored on the surface of sepiolite (Sep) by simple hydrothermal treatment and hydrogenation reduction. The obtained Sep-BFTiO2 nanocomposites showed the dark color, desired crystallinity, and good dispersion, with the great improvement of visible light absorption, photoinduced carriers separation, and bandgap narrowing. The photocatalytic properties of the composites were investigated using rhodamine B (RhB) and tetracycline (TC) as the target pollutants. The results indicate that under visible light irradiation, Sep-BFTiO2 composites showed excellent photodegradation removal toward RhB (91%) and TC (94%), much higher than pure TiO2 toward RhB (22%) and TC (34%), respectively. This study provides a great potential way for the evolution of TiO2 photocatalyst and application of sepiolite in an available and convenient manner.", "title+abstract_embedding_0": 0.48357034, "title+abstract_embedding_1": 1.1387844, "title+abstract_embedding_2": -0.31113723, "title+abstract_embedding_3": 0.39764506, "title+abstract_embedding_4": -0.06750411, "title+abstract_embedding_5": 0.4135748, "title+abstract_embedding_6": -0.30485222, "title+abstract_embedding_7": -0.02289562, "title+abstract_embedding_8": 0.31189895, "title+abstract_embedding_9": 0.008475065, "title+abstract_embedding_10": 0.10562353, "title+abstract_embedding_11": 0.0873597, "title+abstract_embedding_12": -0.21866229, "title+abstract_embedding_13": -0.053760596, "title+abstract_embedding_14": -0.13894968, "title+abstract_embedding_15": 0.09740232, "title+abstract_embedding_16": -0.297843, "title+abstract_embedding_17": 0.33017746, "title+abstract_embedding_18": 0.34804022, "title+abstract_embedding_19": 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"title+abstract_embedding_88": -0.15665312, "title+abstract_embedding_89": -0.008556396, "title+abstract_embedding_90": -0.023391329, "title+abstract_embedding_91": 0.28731886, "title+abstract_embedding_92": 0.17283322, "title+abstract_embedding_93": 0.2342669, "title+abstract_embedding_94": 0.04924178, "title+abstract_embedding_95": 0.34918666, "title+abstract_embedding_96": -0.054475762, "title+abstract_embedding_97": -0.09013898, "title+abstract_embedding_98": -0.091302566, "title+abstract_embedding_99": 0.005185388, "title+abstract_embedding_100": -0.04479538, "title+abstract_embedding_101": 0.1999853, "title+abstract_embedding_102": 0.024730794, "title+abstract_embedding_103": -0.007043317, "title+abstract_embedding_104": 0.016754836, "title+abstract_embedding_105": 0.019357152, "title+abstract_embedding_106": -0.18682522, "title+abstract_embedding_107": -0.20237644, "title+abstract_embedding_108": 0.057775512, "title+abstract_embedding_109": -0.049460202, "title+abstract_embedding_110": 0.14622688, "title+abstract_embedding_111": -0.05610054, "title+abstract_embedding_112": -0.07342829, "title+abstract_embedding_113": 0.11815713, "title+abstract_embedding_114": 0.12728834, "title+abstract_embedding_115": 0.020485826, "title+abstract_embedding_116": -0.17487575, "title+abstract_embedding_117": -0.001732096, "title+abstract_embedding_118": -0.03370972, "title+abstract_embedding_119": 0.052213844, "title+abstract_embedding_120": 0.006724749, "title+abstract_embedding_121": 0.07591271, "title+abstract_embedding_122": -0.08451024, "title+abstract_embedding_123": -0.052199334, "title+abstract_embedding_124": 0.22712776, "title+abstract_embedding_125": 0.14315633, "title+abstract_embedding_126": -0.09108912, "title+abstract_embedding_127": 0.09305097, "label": 3, "label-multi": "1;3;36" }, { "paper_new_id": 174, "id": "j_e360a3232dfdad45d92150a8baa2dbec", "title+abstract": "Facile Fabrication of BiOI/BiOCl Immobilized Films With Improved Visible Light Photocatalytic Performance;HIGHLIGHTS A facial method was used to fabricate BiOI/BiOCl film at room temperature. 30% BiOI/BiOCl showed an excellent photocatalytic activity and stability. Improvement of photocatalytic activity was owed to expanded visible light absorption and high separation efficiency of charge. Photocatalysis has been considered to be one of the most promising ways to photodegrade organic pollutants. Herein, a series of BiOI/BiOCl films coating on FTO were fabricated through a simple method at room temperature. The photocatalytic efficiency of 30%BiOI/BiOCl could reach more than 99% aiming to degrading RhB and MB after 90 and 120 min, respectively. Compared with BiOCl, 30%BiOI/BiOCl showed 12 times higher efficiency when degrading RhB. In comparison with BiOI, 30%BiOI/BiOCl showed 5 and 6 times higher efficiency when degrading RhB and MB, respectively. These obvious enhancements were attributed to expanded visible light absorption and high separation performance of photoinduced charge. Moreover, the photocatalytic activity of 30%BiOI/BiOCl had no obvious decrease after five recycles, suggesting that it was a promising photocatalyst for the removal of MB and RhB pollutants. Finally, the possible growth process for the BiOI/BiOCl thin films and photocatalysis mechanism were investigated in details. This work would provide insight to the reasonable construction of BiOX heterojunction and the photocatalytic mechanism in degrading organic pollutants.", "title+abstract_embedding_0": 0.6723803, "title+abstract_embedding_1": 0.7799263, "title+abstract_embedding_2": 0.34074202, "title+abstract_embedding_3": 0.05940956, "title+abstract_embedding_4": -0.44509724, "title+abstract_embedding_5": -0.030792475, "title+abstract_embedding_6": -0.74651694, "title+abstract_embedding_7": -0.32892355, "title+abstract_embedding_8": -0.109306395, "title+abstract_embedding_9": -0.16550899, "title+abstract_embedding_10": -0.015572816, "title+abstract_embedding_11": 0.5790458, "title+abstract_embedding_12": -0.081707925, "title+abstract_embedding_13": 0.14673337, "title+abstract_embedding_14": -0.14092308, "title+abstract_embedding_15": 0.21187061, "title+abstract_embedding_16": 0.018239409, "title+abstract_embedding_17": -0.1665563, "title+abstract_embedding_18": 0.2775578, 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-0.19322525, "title+abstract_embedding_110": -0.04024981, "title+abstract_embedding_111": -0.15013658, "title+abstract_embedding_112": -0.17198493, "title+abstract_embedding_113": -0.055539608, "title+abstract_embedding_114": 0.08606903, "title+abstract_embedding_115": -0.12605035, "title+abstract_embedding_116": -0.08560319, "title+abstract_embedding_117": -0.050383277, "title+abstract_embedding_118": -0.047701538, "title+abstract_embedding_119": 0.043059833, "title+abstract_embedding_120": -0.006548499, "title+abstract_embedding_121": -0.038016148, "title+abstract_embedding_122": -0.222637, "title+abstract_embedding_123": 0.2193071, "title+abstract_embedding_124": 0.2825398, "title+abstract_embedding_125": -0.051392667, "title+abstract_embedding_126": -0.02674465, "title+abstract_embedding_127": 0.14877038, "label": 3, "label-multi": "3" }, { "paper_new_id": 175, "id": "j_e36666e90b4a7c1dd1308b7fa8e22ce7", "title+abstract": "Efficient photo-Fenton activity in mesoporous MIL-100(Fe) decorated with ZnO nanosphere for pollutants degradation;Abstract Metal-organic frameworks (MOFs) have received significant interest as a promising photocatalyst for environmental remediation due to its high surface area and porous nature. The small pores ( 2?nm) and open pore cavities that can provide right pathways for ingoing and outgoing of molecules during catalysis. Herein, we successfully report stable mesoporous MIL-100(Fe) loaded with ZnO NS by an in situ self-assembly method. The prepared samples were characterized by Brunauer¡§CEmmett¡§CTeller (BET) and N2 adsorption-desorption isotherm to study their surface area and porosity. The catalytic performance of mesoporous MIL-100(Fe) was approximately 2¡§C3 order of magnitude more than that of microporous MIL-100(Fe). Such higher catalytic activity in mesoporous MIL-100(Fe) can be ascribed to its mesocellular structure which can improve the molecular diffusion and accessibility inside MOF channels. The charge separation efficiency and photo-Fenton activity of mesoporous MIL-100(Fe) can further be increased by introduction of certain amount of ZnO NS and H2O2. Moreover, the as synthesized sample shows higher photo-Fenton degradation efficiency at lower pH value with certain amount of H2O2. Lastly, the possible catalytic mechanism has been tentatively proposed. This study not only used for the pollutants degradation but also provide useful platform for the application of mesoporous MOFs as an efficient photo-Fenton activity to various other fields.", "title+abstract_embedding_0": 0.77435744, "title+abstract_embedding_1": -0.10545336, "title+abstract_embedding_2": -0.08331379, "title+abstract_embedding_3": -0.4363693, "title+abstract_embedding_4": -0.010897756, "title+abstract_embedding_5": -0.42981386, "title+abstract_embedding_6": -0.5028844, "title+abstract_embedding_7": 0.23069821, "title+abstract_embedding_8": 0.03907803, "title+abstract_embedding_9": 0.40798062, "title+abstract_embedding_10": -0.06266689, "title+abstract_embedding_11": 0.08428112, "title+abstract_embedding_12": -0.04721248, "title+abstract_embedding_13": 0.02981896, "title+abstract_embedding_14": 0.085664034, "title+abstract_embedding_15": -0.15760137, "title+abstract_embedding_16": 0.009415001, "title+abstract_embedding_17": -0.2796718, "title+abstract_embedding_18": 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"title+abstract_embedding_109": 0.007316425, "title+abstract_embedding_110": 0.014015555, "title+abstract_embedding_111": -0.030833507, "title+abstract_embedding_112": -0.07135658, "title+abstract_embedding_113": 0.17041054, "title+abstract_embedding_114": 0.037234873, "title+abstract_embedding_115": -0.08411562, "title+abstract_embedding_116": 0.10815078, "title+abstract_embedding_117": -0.12714806, "title+abstract_embedding_118": -0.017861638, "title+abstract_embedding_119": 0.04161282, "title+abstract_embedding_120": -0.061712373, "title+abstract_embedding_121": 0.1072912, "title+abstract_embedding_122": 0.1383581, "title+abstract_embedding_123": 0.1097761, "title+abstract_embedding_124": 0.11383011, "title+abstract_embedding_125": -0.028462708, "title+abstract_embedding_126": 0.045226254, "title+abstract_embedding_127": -0.20447612, "label": 3, "label-multi": "0;3" }, { "paper_new_id": 176, "id": "j_e4d32584ed7f1e0d6199a130d61a2a96", "title+abstract": "Counter electrodes from polymorphic platinum-nickel hollow alloys for high-efficiency dye-sensitized solar cells;Precious platinum counter electrode (CE) has been an economic burden for future commercialization of dye-sensitized solar cells (DSSCs). Low-platinum alloy CE catalysts are promising in bringing down the solar cell cost without reducing photovoltaic performances. We present here a facile strategy of fabricating ZnO nanorods assisted platinum-nickel (PtNi) alloy microtube CEs for liquid junction DSSCs. By adjusting the concentration of zinc precursors, the ZnO nanostructures and therefore PtNi alloys are optimized to maximize the electrocatalytic behaviors toward triiodide reduction reaction. The maximal power conversion efficiency is determined as high as 8.43% for liquid junction DSSC device with alloyed PtNi microtube CE synthesized at 75 mM Zn(NO3)(2) aqueous solution, yielding a 32.8% enhancement in cell efficiency in comparison with the solar cell from pristine platinum electrode. Moreover, the dissolution resistance and charge-transfer ability toward redox couples have also been markedly enhanced due to competitive dissolution reactions and alloyed effects. (C) 2016 Elsevier B.V. All rights reserved.", "title+abstract_embedding_0": -0.33179414, "title+abstract_embedding_1": -0.3778865, "title+abstract_embedding_2": -0.886431, "title+abstract_embedding_3": 0.18910229, "title+abstract_embedding_4": 0.06924176, "title+abstract_embedding_5": -0.4614458, "title+abstract_embedding_6": -0.013266951, "title+abstract_embedding_7": -0.289699, "title+abstract_embedding_8": 0.8993077, "title+abstract_embedding_9": -0.55277216, "title+abstract_embedding_10": -0.3706478, "title+abstract_embedding_11": 0.05375494, "title+abstract_embedding_12": 0.607998, "title+abstract_embedding_13": -0.41987768, "title+abstract_embedding_14": -0.6071221, "title+abstract_embedding_15": 0.22490954, "title+abstract_embedding_16": -0.47150797, "title+abstract_embedding_17": -0.06808743, "title+abstract_embedding_18": 0.38972712, "title+abstract_embedding_19": -0.5939827, "title+abstract_embedding_20": 0.09500058, "title+abstract_embedding_21": 0.13971531, "title+abstract_embedding_22": 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"title+abstract_embedding_112": -0.00907138, "title+abstract_embedding_113": -0.20854317, "title+abstract_embedding_114": 0.07231437, "title+abstract_embedding_115": 0.08094982, "title+abstract_embedding_116": 0.023488335, "title+abstract_embedding_117": 0.004879855, "title+abstract_embedding_118": 0.10338504, "title+abstract_embedding_119": 0.03796175, "title+abstract_embedding_120": 0.078422636, "title+abstract_embedding_121": 0.066895306, "title+abstract_embedding_122": -0.045748055, "title+abstract_embedding_123": 0.11989396, "title+abstract_embedding_124": 0.0717071, "title+abstract_embedding_125": 0.079832844, "title+abstract_embedding_126": -0.07444654, "title+abstract_embedding_127": 0.049334273, "label": 3, "label-multi": "1;14;17;3" }, { "paper_new_id": 177, "id": "j_e56ca7fae152ed9c9fccf643eb377553", "title+abstract": "Fabrication of efficient CuO / graphitic carbon nitride based heterogeneous photo-Fenton like catalyst for degradation of 2, 4 dimethyl phenol;Abstract Considering the drawbacks of iron-based Fenton process, this work was aimed at designing of an efficient photo-Fenton like process via coupling of CuO/g-C3N4 photocatalyst with H2O2. The photo-Fenton like catalytic process was used for degradation of 2, 4-dimethyl phenol (DMP). The X% CuO/g-C3N4 Z-shceme photocatalyst samples were fabricated by thermal calcination method, varing the CuO percentage (X = 2 %, 4 % and 8 %) loaded on g-C3N4. A lab-scale photoreactor was used to assess and select the optimal removal efficiency for DMP degradation. The photocatalyst was characterized by advanced spectral techniques. Coupling of CuO/GCN system with H2O2 significantly improved photocatalytic activity via photo-Fenton process. The kinetics of photo-degradation was found to exhibit pseudo-first order reaction rules. The rate of photodegradation was strongly influenced by pH and different concentrations of H2O2. 4%CuO/g-C3N4/H2O2 system proved to be the most efficient and exhibited much higher photo removal efficiency than CuO/g-C3N4 system and permitted attaining 99 % degradation of DMP in reaction time of 120 min. The successful implementation of this work was effective and of significance for the economical decomposition process of pollutants present in water under visible light irradiation. Overall, utilization of the studied system leads to high catalytic efficiency in a relatively short degradation period, which is of immense potential in water purification.", "title+abstract_embedding_0": 0.49002624, "title+abstract_embedding_1": 1.0610073, "title+abstract_embedding_2": 0.6323586, "title+abstract_embedding_3": -0.37180662, "title+abstract_embedding_4": 0.24358779, "title+abstract_embedding_5": -0.5581522, "title+abstract_embedding_6": -0.6327565, "title+abstract_embedding_7": -0.32718313, "title+abstract_embedding_8": -0.03373173, "title+abstract_embedding_9": -0.23298728, "title+abstract_embedding_10": -0.20772102, "title+abstract_embedding_11": 0.11861324, "title+abstract_embedding_12": -0.260668, "title+abstract_embedding_13": 0.47186258, "title+abstract_embedding_14": 0.0885337, "title+abstract_embedding_15": 0.033077683, "title+abstract_embedding_16": 0.020192474, "title+abstract_embedding_17": -0.1399062, "title+abstract_embedding_18": -0.22798169, 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Microperoxidase-11 and Nitrate Reductase Monolayer on a Gold Electrode: An Integrated Electrically Contacted Electrode for the Bioelectrocatalyzed Reduction of NO3a??;nan", "title+abstract_embedding_0": -2.0782235, "title+abstract_embedding_1": -0.39323595, "title+abstract_embedding_2": -0.42465004, "title+abstract_embedding_3": 0.02101487, "title+abstract_embedding_4": -0.013228357, "title+abstract_embedding_5": -0.8768356, "title+abstract_embedding_6": 0.06530905, "title+abstract_embedding_7": 0.2284359, "title+abstract_embedding_8": -0.8088758, "title+abstract_embedding_9": -0.43067157, "title+abstract_embedding_10": 0.062356174, "title+abstract_embedding_11": 0.7135957, "title+abstract_embedding_12": -0.09875435, "title+abstract_embedding_13": 0.3756221, "title+abstract_embedding_14": -0.5300945, "title+abstract_embedding_15": 0.002012714, "title+abstract_embedding_16": 0.044558406, "title+abstract_embedding_17": 1.0528948, "title+abstract_embedding_18": 0.28376853, 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"title+abstract_embedding_88": -0.16795972, "title+abstract_embedding_89": 0.33157918, "title+abstract_embedding_90": 0.24033958, "title+abstract_embedding_91": -0.054712497, "title+abstract_embedding_92": -0.004568823, "title+abstract_embedding_93": -0.16154335, "title+abstract_embedding_94": -0.003522724, "title+abstract_embedding_95": -0.31966287, "title+abstract_embedding_96": -0.111963175, "title+abstract_embedding_97": -0.08046753, "title+abstract_embedding_98": 0.040704794, "title+abstract_embedding_99": -0.100044236, "title+abstract_embedding_100": 0.050084785, "title+abstract_embedding_101": -0.080990046, "title+abstract_embedding_102": 0.015189108, "title+abstract_embedding_103": 0.09447512, "title+abstract_embedding_104": 0.11266885, "title+abstract_embedding_105": -0.24077082, "title+abstract_embedding_106": 0.19496779, "title+abstract_embedding_107": -0.0438674, "title+abstract_embedding_108": 0.12642191, "title+abstract_embedding_109": 0.07494654, "title+abstract_embedding_110": 0.082347184, "title+abstract_embedding_111": -0.045218825, "title+abstract_embedding_112": 0.17353621, "title+abstract_embedding_113": -0.10530536, "title+abstract_embedding_114": -0.1592079, "title+abstract_embedding_115": -0.1291973, "title+abstract_embedding_116": -0.14761426, "title+abstract_embedding_117": 0.013569389, "title+abstract_embedding_118": 0.04700313, "title+abstract_embedding_119": -0.17021689, "title+abstract_embedding_120": -0.294931, "title+abstract_embedding_121": -0.010536058, "title+abstract_embedding_122": -0.09536958, "title+abstract_embedding_123": -0.056698985, "title+abstract_embedding_124": -0.010502264, "title+abstract_embedding_125": -0.008947678, "title+abstract_embedding_126": -0.18975797, "title+abstract_embedding_127": 0.05089467, "label": 3, "label-multi": "3" }, { "paper_new_id": 179, "id": "j_e605986029a722ba53a7af12a3a4e414", "title+abstract": "Stable single-atom cobalt as a strong coupling bridge to promote electron transfer and separation in photoelectrocatalysis;In photoelectrochemical water decomposition field, it remains a key challenge to develop photoanodes with excellent charge separation and transfer, efficient solar collection and rapid surface reaction kinetics. Here, we report a new strongly coupled ternary hybrid system using a single atom as a \"bridge\" to achieve high efficiency water oxidation photoelectrochemical performance, by constructing a monoatomic transition metal tightly bound to the core-shell gap which formed by lamina g-C3N4 coating on the surface of porous carbon balls. Experimental results and density functional theory calculations show that the unique structure combines lots of beneficial features, that is efficient light trapping and photo generated charge separation, strong coupling effects, fast electron transport paths and improved surface reaction dynamics. Benefited from the ideal nanostructure, the photocurrent density reached 5.08 mA cm(-2) at 1.23 V and the IPCE value achieved 27.5% at 350 nm under AM 1.5 G illumination. This work has promoted a significant step of developing single-atom photoanodes with unique structure for solar water splitting, as well as the design of thermochemically stable catalysts. (C) 2019 Elsevier Inc. All rights reserved.", "title+abstract_embedding_0": -0.22169507, "title+abstract_embedding_1": 0.33209217, "title+abstract_embedding_2": -0.21904138, "title+abstract_embedding_3": -0.6472539, "title+abstract_embedding_4": -0.3639025, "title+abstract_embedding_5": 0.0744738, "title+abstract_embedding_6": 0.40632308, "title+abstract_embedding_7": -0.58674526, "title+abstract_embedding_8": -0.04681802, "title+abstract_embedding_9": -0.38691407, "title+abstract_embedding_10": -0.11996509, "title+abstract_embedding_11": -0.28618425, "title+abstract_embedding_12": -0.5040543, "title+abstract_embedding_13": -0.046496022, "title+abstract_embedding_14": 0.51775527, "title+abstract_embedding_15": 0.186676, "title+abstract_embedding_16": -0.17214553, "title+abstract_embedding_17": 0.27073333, "title+abstract_embedding_18": 0.44011253, "title+abstract_embedding_19": -0.23251113, "title+abstract_embedding_20": -0.089209065, "title+abstract_embedding_21": -0.031597737, 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"title+abstract_embedding_112": -0.018845126, "title+abstract_embedding_113": -0.029883146, "title+abstract_embedding_114": -0.14877328, "title+abstract_embedding_115": 0.0748026, "title+abstract_embedding_116": 0.006846003, "title+abstract_embedding_117": -0.13344774, "title+abstract_embedding_118": 0.19330586, "title+abstract_embedding_119": 0.053419884, "title+abstract_embedding_120": -0.006547512, "title+abstract_embedding_121": 0.11229995, "title+abstract_embedding_122": 0.11299887, "title+abstract_embedding_123": -0.013634875, "title+abstract_embedding_124": 0.020940132, "title+abstract_embedding_125": 0.08363915, "title+abstract_embedding_126": 0.1414846, "title+abstract_embedding_127": 0.002340674, "label": 106, "label-multi": NaN }, { "paper_new_id": 180, "id": "j_e60c1cf436e102b400c3ab5332845d30", "title+abstract": "The role of ruthenium photosensitizers in the degradation of phenazopyridine with TiO2 electrospun fibers;Abstract There has been increased interest in titanium dioxide (TiO2) fibers as a photocatalyst for the degradation of persistent organic and biopharmaceutical toxins in the environment. The photocatalytic efficiency of TiO2 fibers is typically limited to UV irradiation due to its semiconductor bandgap. TiO2 fibers have been prepared and adsorbed the visible photosensitizer cis-dichlorobis(2,2??-bipyridyl-4,4??-dicarboxylic acid)ruthenium (II) (Ru(dcbpyH2)2Cl2) on the surface in order to absorb from 300 to 800?nm in the visible spectrum and drive photocatalysis. This dye fiber material has been applied to the degradation of 2,6-pyridinediamine,3-(phenylazo) monohydrochloride or phenazopyridine (PAP) as a model biopharmaceutical waste. The Ru(dcbpyH2)2Cl2¡§Csensitized fibers degrade PAP under UV and visible irradiation following a first order reaction rate. The rate constants for PAP degradation in visible light when using bare TiO2 fibers and dye-sensitized TiO2 fibers were 0.014??¨¤?0.001?min?1 and 0.012??¨¤?0.001?min?1 respectively, showing little change. Under UV irradiation, the rate decreased from 0.032??¨¤?0.003?min?1 and 0.012??¨¤?0.002?min?1. These results suggest that the major pathway for the degradation of PAP may occur through the valence band.", "title+abstract_embedding_0": 1.1430243, "title+abstract_embedding_1": 0.94978774, "title+abstract_embedding_2": 0.6194236, "title+abstract_embedding_3": 0.6771143, "title+abstract_embedding_4": 0.22431546, "title+abstract_embedding_5": -0.27967602, "title+abstract_embedding_6": -0.08088577, "title+abstract_embedding_7": 0.10590056, "title+abstract_embedding_8": -0.10239582, "title+abstract_embedding_9": -0.32795256, "title+abstract_embedding_10": -0.19348907, "title+abstract_embedding_11": -0.374848, "title+abstract_embedding_12": 0.08857003, "title+abstract_embedding_13": 0.04195714, "title+abstract_embedding_14": -0.34117785, "title+abstract_embedding_15": 0.0953122, "title+abstract_embedding_16": -0.32539862, "title+abstract_embedding_17": 0.058508307, "title+abstract_embedding_18": -0.22874464, "title+abstract_embedding_19": 0.003490003, "title+abstract_embedding_20": 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"title+abstract_embedding_43": 0.050612643, "title+abstract_embedding_44": 0.105028614, "title+abstract_embedding_45": -0.1635536, "title+abstract_embedding_46": 0.006419748, "title+abstract_embedding_47": -0.25418007, "title+abstract_embedding_48": 0.18908948, "title+abstract_embedding_49": 0.09112911, "title+abstract_embedding_50": 0.013347913, "title+abstract_embedding_51": -0.1310992, "title+abstract_embedding_52": -0.10082475, "title+abstract_embedding_53": 0.12429577, "title+abstract_embedding_54": -0.057990603, "title+abstract_embedding_55": 0.23537178, "title+abstract_embedding_56": -0.075087026, "title+abstract_embedding_57": -0.2730034, "title+abstract_embedding_58": 0.18602358, "title+abstract_embedding_59": -0.13800336, "title+abstract_embedding_60": 0.1437609, "title+abstract_embedding_61": 0.31531993, "title+abstract_embedding_62": -0.107153945, "title+abstract_embedding_63": 0.043914206, "title+abstract_embedding_64": 0.033205286, "title+abstract_embedding_65": 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"title+abstract_embedding_88": -0.079529464, "title+abstract_embedding_89": -0.12029139, "title+abstract_embedding_90": -0.10975657, "title+abstract_embedding_91": -0.08745272, "title+abstract_embedding_92": 0.03211791, "title+abstract_embedding_93": -0.07434858, "title+abstract_embedding_94": -0.066916004, "title+abstract_embedding_95": -0.053678617, "title+abstract_embedding_96": -0.043727525, "title+abstract_embedding_97": 0.2945633, "title+abstract_embedding_98": -0.07324422, "title+abstract_embedding_99": 0.1112246, "title+abstract_embedding_100": -0.048973158, "title+abstract_embedding_101": -0.045955107, "title+abstract_embedding_102": -0.04898782, "title+abstract_embedding_103": 0.09965983, "title+abstract_embedding_104": -0.01906085, "title+abstract_embedding_105": 0.2447962, "title+abstract_embedding_106": -0.0432982, "title+abstract_embedding_107": 0.11493761, "title+abstract_embedding_108": -0.174436, "title+abstract_embedding_109": -0.007207081, "title+abstract_embedding_110": 0.06045407, "title+abstract_embedding_111": -0.042945497, "title+abstract_embedding_112": 0.08069673, "title+abstract_embedding_113": 0.025048062, "title+abstract_embedding_114": -0.04308165, "title+abstract_embedding_115": -0.106177874, "title+abstract_embedding_116": 0.1710522, "title+abstract_embedding_117": 0.10251193, "title+abstract_embedding_118": -0.07986209, "title+abstract_embedding_119": -0.05681295, "title+abstract_embedding_120": -0.091648445, "title+abstract_embedding_121": -0.03118725, "title+abstract_embedding_122": -0.09239492, "title+abstract_embedding_123": -0.032216962, "title+abstract_embedding_124": -0.19843549, "title+abstract_embedding_125": -0.023279697, "title+abstract_embedding_126": -0.28398696, "title+abstract_embedding_127": 0.056224316, "label": 3, "label-multi": "3" }, { "paper_new_id": 181, "id": "j_e6d87981091303d025083f53a85bcf5e", "title+abstract": "Highly sensitive and selective serotonin sensor based on gamma ray irradiated tungsten trioxide nanoparticles;Abstract This work investigates the sensitive and selective electrochemical method for determining serotonin (5-HT) using gamma ray irradiated tungsten trioxide (GI-WO 3 ) nanoparticles. WO 3 NPs synthesized by microwave irradiation method was subjected to gamma ray irradiation under different doses (0¡§C150?kGy) and the products were characterized by powder XRD, HRTEM, Raman and UV¡§Cvis spectra. The experimental results demonstrated that the 100 kGy irradiation on WO 3 NPs led to significant changes in morphology, crystal structure and improvement in specific surface area and fast electron transfer rate which enhanced its electrocatalytic activity greatly. Cyclic voltammetry and differential pulse voltammetry studies of GI-WO 3 NPs modified glassy carbon electrodes (GCE) exhibited improved electrocatalytic activity towards the oxidation of 5-HT in a phosphate buffer solution (PBS, pH 7.0). The kinetic parameters such as diffusion coefficient, electron transfer coefficient and heterogeneous electron transfer rate constant involved in the oxidation of 5-HT at the 100 kGy GI-WO 3 /GCE indicate the suitability of the fabricated electrode for the detection of 5-HT. Under the optimized conditions, the oxidation peak currents were linearly proportional to 5-HT concentration over a wide linear range of 0.01¡§C600?|¨¬M, with the lowest detection limit of 1.42?nM (S/N?=?3). The fabricated 5-HT sensor showed an excellent anti-interference ability against potentially coexisting electroactive species, long-term high stability and excellent reproducibility. The proposed sensor was successfully implemented for the determination of 5-HT in human blood serum samples with good recoveries ranging from 99.2% and 102.9%.", "title+abstract_embedding_0": 0.9088205, "title+abstract_embedding_1": -1.1038077, "title+abstract_embedding_2": -0.18946114, "title+abstract_embedding_3": 0.10863286, "title+abstract_embedding_4": -0.26569718, "title+abstract_embedding_5": -0.5142505, "title+abstract_embedding_6": 0.17877387, "title+abstract_embedding_7": -0.07599749, "title+abstract_embedding_8": -0.33694026, "title+abstract_embedding_9": -0.21784717, "title+abstract_embedding_10": 0.12000862, "title+abstract_embedding_11": 0.3453005, "title+abstract_embedding_12": 0.06775029, "title+abstract_embedding_13": -0.15864986, "title+abstract_embedding_14": -0.2500119, "title+abstract_embedding_15": 0.1416797, "title+abstract_embedding_16": -0.05663225, "title+abstract_embedding_17": 0.32211384, "title+abstract_embedding_18": -0.002625167, "title+abstract_embedding_19": -0.07637651, "title+abstract_embedding_20": -0.3838432, "title+abstract_embedding_21": 0.2302455, "title+abstract_embedding_22": 0.116502225, "title+abstract_embedding_23": -0.088906825, "title+abstract_embedding_24": -0.18376616, "title+abstract_embedding_25": -0.1836622, "title+abstract_embedding_26": -0.120498866, "title+abstract_embedding_27": -0.11576994, "title+abstract_embedding_28": 0.27659792, "title+abstract_embedding_29": 0.40020943, "title+abstract_embedding_30": -0.02682425, "title+abstract_embedding_31": -0.06999477, "title+abstract_embedding_32": -0.15769926, "title+abstract_embedding_33": -0.42238417, "title+abstract_embedding_34": 0.23296604, "title+abstract_embedding_35": -0.22537446, "title+abstract_embedding_36": -0.20893037, "title+abstract_embedding_37": 0.17617725, "title+abstract_embedding_38": 0.32243988, "title+abstract_embedding_39": 0.22312072, "title+abstract_embedding_40": 0.031243056, "title+abstract_embedding_41": 0.109959885, "title+abstract_embedding_42": -0.34337422, "title+abstract_embedding_43": 0.40047544, "title+abstract_embedding_44": 0.002879411, "title+abstract_embedding_45": -0.0544084, "title+abstract_embedding_46": 0.37334368, "title+abstract_embedding_47": -0.012781125, "title+abstract_embedding_48": 0.05134186, "title+abstract_embedding_49": 0.21458435, "title+abstract_embedding_50": -0.18687901, "title+abstract_embedding_51": -0.003246114, "title+abstract_embedding_52": 0.06861617, "title+abstract_embedding_53": 0.2039818, "title+abstract_embedding_54": -0.10179955, "title+abstract_embedding_55": -0.24020095, "title+abstract_embedding_56": 0.3469948, "title+abstract_embedding_57": 0.008729652, "title+abstract_embedding_58": 0.15243284, "title+abstract_embedding_59": -0.10688777, "title+abstract_embedding_60": 0.006900877, "title+abstract_embedding_61": 0.06675957, "title+abstract_embedding_62": -0.10583139, "title+abstract_embedding_63": 0.024152506, "title+abstract_embedding_64": -0.052046195, "title+abstract_embedding_65": 0.068751976, "title+abstract_embedding_66": 0.098694965, "title+abstract_embedding_67": -0.12988639, "title+abstract_embedding_68": -0.18980044, "title+abstract_embedding_69": -0.21191344, "title+abstract_embedding_70": 0.13780059, "title+abstract_embedding_71": -0.17314926, "title+abstract_embedding_72": -0.10179024, "title+abstract_embedding_73": -0.056161013, "title+abstract_embedding_74": -0.15667473, "title+abstract_embedding_75": 0.15652707, "title+abstract_embedding_76": 0.20207392, "title+abstract_embedding_77": -0.054788485, "title+abstract_embedding_78": -0.017503679, "title+abstract_embedding_79": -0.12131545, "title+abstract_embedding_80": 0.16257703, "title+abstract_embedding_81": 0.030642036, "title+abstract_embedding_82": -0.03291905, "title+abstract_embedding_83": -0.051564105, "title+abstract_embedding_84": 0.11726538, "title+abstract_embedding_85": 0.05944766, "title+abstract_embedding_86": -0.12945443, "title+abstract_embedding_87": -0.06952631, "title+abstract_embedding_88": 0.10934535, "title+abstract_embedding_89": -0.069464676, "title+abstract_embedding_90": -0.014912166, "title+abstract_embedding_91": 0.050286487, "title+abstract_embedding_92": -0.09130456, "title+abstract_embedding_93": -0.11474119, "title+abstract_embedding_94": -0.12455909, "title+abstract_embedding_95": 0.022937268, "title+abstract_embedding_96": 0.17337501, "title+abstract_embedding_97": -0.04510954, "title+abstract_embedding_98": 0.023447365, "title+abstract_embedding_99": -0.02670683, "title+abstract_embedding_100": 0.059141222, "title+abstract_embedding_101": 0.07787964, "title+abstract_embedding_102": -0.09568285, "title+abstract_embedding_103": 0.14763305, "title+abstract_embedding_104": -0.23401195, "title+abstract_embedding_105": 0.17292349, "title+abstract_embedding_106": 0.08360597, "title+abstract_embedding_107": -0.026486851, "title+abstract_embedding_108": -0.04183291, "title+abstract_embedding_109": 0.12367956, "title+abstract_embedding_110": -0.06902148, "title+abstract_embedding_111": -0.07538442, "title+abstract_embedding_112": -0.08799155, "title+abstract_embedding_113": -0.10216907, "title+abstract_embedding_114": -0.08093369, "title+abstract_embedding_115": 0.07586149, "title+abstract_embedding_116": 0.10294659, "title+abstract_embedding_117": 0.05245101, "title+abstract_embedding_118": -0.017821498, "title+abstract_embedding_119": -0.044848762, "title+abstract_embedding_120": -0.06659228, "title+abstract_embedding_121": 0.033478603, "title+abstract_embedding_122": -0.027845323, "title+abstract_embedding_123": -0.08893875, "title+abstract_embedding_124": -0.047231786, "title+abstract_embedding_125": 0.025481347, "title+abstract_embedding_126": 0.012030169, "title+abstract_embedding_127": 0.121956855, "label": 3, "label-multi": "14;24;3" }, { "paper_new_id": 182, "id": "j_e8aed88f6ed632ee8beef68a4462e6a2", "title+abstract": "Enhanced Pt utilization in electrocatalysts by covering of colloidal silica nanoparticles;Abstract This work aims at enhancing Pt utilization in electrocatalysts by covering of preformed silica nanoparticles. Pt/C electrocatalysts were prepared by reductive deposition of Pt by citrate at moderate temperatures on silica nanoparticles with varying atomic silica to Pt ratios (1.7:1 and 3.3:1) to study the effects of silica to Pt ratio. Considerable voidages were created by inter-situated 10¡§C20?nm silica nanoparticles between support carbon particulates to facilitate mass transfer of reactants and products. This particular method of catalyst preparation increases the Pt metal utilization, and generates a large amount of accessible voidage in the interpenetrating particle network of carbon and silica to support the facile transport of reactants and products. Electrochemical hydrogen adsorption/desorption has shown an increase in electrochemically active surface area by this approach. Methanol electro-oxidation was used as a test reaction to evaluate the catalytic activity. It was found that the Pt catalyst modified with silica at silica:Pt?=?1.7:1 atomic ratio was more active than a catalyst prepared when silica to Pt ratio increased to 3.3:1.", "title+abstract_embedding_0": -0.003663182, "title+abstract_embedding_1": -0.5960364, "title+abstract_embedding_2": -0.36188057, "title+abstract_embedding_3": 0.15214819, "title+abstract_embedding_4": 0.80095893, "title+abstract_embedding_5": 0.5062112, "title+abstract_embedding_6": -0.17913273, "title+abstract_embedding_7": 0.085112326, "title+abstract_embedding_8": 0.38853437, "title+abstract_embedding_9": -0.64865696, "title+abstract_embedding_10": -0.13290139, "title+abstract_embedding_11": 0.268709, "title+abstract_embedding_12": 0.56323344, "title+abstract_embedding_13": 0.19703433, "title+abstract_embedding_14": -0.2868798, "title+abstract_embedding_15": 0.17542309, "title+abstract_embedding_16": 0.59124386, "title+abstract_embedding_17": -0.029688835, "title+abstract_embedding_18": -0.17647994, "title+abstract_embedding_19": -0.044260915, "title+abstract_embedding_20": 0.16170488, "title+abstract_embedding_21": 0.019856758, "title+abstract_embedding_22": -0.019206801, "title+abstract_embedding_23": -0.22164917, "title+abstract_embedding_24": 0.0742973, "title+abstract_embedding_25": 0.22519463, "title+abstract_embedding_26": 0.21514377, "title+abstract_embedding_27": -0.048982393, "title+abstract_embedding_28": 0.00091733, "title+abstract_embedding_29": 0.35180473, "title+abstract_embedding_30": 0.25700435, "title+abstract_embedding_31": -0.16347888, "title+abstract_embedding_32": -0.19059217, "title+abstract_embedding_33": -0.041899472, "title+abstract_embedding_34": 0.13477886, "title+abstract_embedding_35": -0.06552856, "title+abstract_embedding_36": -0.09394502, "title+abstract_embedding_37": 0.3873812, "title+abstract_embedding_38": 0.057447597, "title+abstract_embedding_39": 0.2742183, "title+abstract_embedding_40": -0.11411542, "title+abstract_embedding_41": 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"title+abstract_embedding_64": -0.02366051, "title+abstract_embedding_65": 0.20363657, "title+abstract_embedding_66": 0.07382086, "title+abstract_embedding_67": 0.0844056, "title+abstract_embedding_68": 0.037709028, "title+abstract_embedding_69": 0.1824202, "title+abstract_embedding_70": -0.06480806, "title+abstract_embedding_71": 0.1321794, "title+abstract_embedding_72": 0.06519753, "title+abstract_embedding_73": 0.10789824, "title+abstract_embedding_74": 0.070455514, "title+abstract_embedding_75": -0.0765445, "title+abstract_embedding_76": -0.11419302, "title+abstract_embedding_77": 0.17741369, "title+abstract_embedding_78": 0.029592767, "title+abstract_embedding_79": 0.09864208, "title+abstract_embedding_80": -0.15529776, "title+abstract_embedding_81": -0.3025083, "title+abstract_embedding_82": 0.12673198, "title+abstract_embedding_83": -0.003618347, "title+abstract_embedding_84": 0.013025537, "title+abstract_embedding_85": 0.15892021, "title+abstract_embedding_86": 0.049246073, "title+abstract_embedding_87": 0.07985991, "title+abstract_embedding_88": -0.055885047, "title+abstract_embedding_89": 0.28519228, "title+abstract_embedding_90": -0.036202617, "title+abstract_embedding_91": -0.05340436, "title+abstract_embedding_92": 0.061181083, "title+abstract_embedding_93": -0.22754845, "title+abstract_embedding_94": 0.04067421, "title+abstract_embedding_95": -0.10654122, "title+abstract_embedding_96": 0.029510386, "title+abstract_embedding_97": 0.012412215, "title+abstract_embedding_98": -0.020536814, "title+abstract_embedding_99": 0.011852503, "title+abstract_embedding_100": 0.00486245, "title+abstract_embedding_101": 0.11678095, "title+abstract_embedding_102": -0.052715734, "title+abstract_embedding_103": 0.0578451, "title+abstract_embedding_104": -0.0406508, "title+abstract_embedding_105": 0.08055571, "title+abstract_embedding_106": 0.10632969, "title+abstract_embedding_107": 0.006670188, "title+abstract_embedding_108": -0.06613755, "title+abstract_embedding_109": -0.012910649, "title+abstract_embedding_110": 0.05157602, "title+abstract_embedding_111": -0.060935557, "title+abstract_embedding_112": -0.028524771, "title+abstract_embedding_113": 0.09366592, "title+abstract_embedding_114": -0.058339447, "title+abstract_embedding_115": -0.04304249, "title+abstract_embedding_116": -0.032961704, "title+abstract_embedding_117": 0.11527612, "title+abstract_embedding_118": 0.076314844, "title+abstract_embedding_119": 0.12396094, "title+abstract_embedding_120": -0.00991056, "title+abstract_embedding_121": 0.13425893, "title+abstract_embedding_122": 0.23103145, "title+abstract_embedding_123": -0.14339037, "title+abstract_embedding_124": -0.009564295, "title+abstract_embedding_125": -0.17456624, "title+abstract_embedding_126": -0.012596353, "title+abstract_embedding_127": -0.022960603, "label": 3, "label-multi": "1;14;17;3" }, { "paper_new_id": 183, "id": "j_e8d9d384e709945b3699c0bfa263c479", "title+abstract": "Photomineralisation of 4-chlorophenol sensitised by titanium dioxide: a study of the effect of annealing the photocatalyst at different temperatures;Abstract The results of a study of the variation in photocatalytic activity of TiO 2 , as measured by its ability to photomineralise 4-chlorophenol, as a function of temperature used to anneal the TiO 2 , are reported. Heat treatment of the TiO 2 leads to a marked decrease in its photocatalytic activity at annealing temperatures above 600??C. This decrease is associated with a concomitant drop in the specific surface area of the TiO 2 , owing to particle sintering, rather than the anatase to rutile transformation, which occurs largely at temperatures above 700??C. There is a reasonable correlation between photocatalytic activity and the surface area of the aggregate particles in the dispersions of the different heat-treated TiO 2 samples.", "title+abstract_embedding_0": 0.33689845, "title+abstract_embedding_1": 1.1283092, "title+abstract_embedding_2": 0.37405258, "title+abstract_embedding_3": 0.7936706, "title+abstract_embedding_4": 0.56050736, "title+abstract_embedding_5": 0.39014465, "title+abstract_embedding_6": 0.44286644, "title+abstract_embedding_7": 0.06297148, "title+abstract_embedding_8": -0.20872615, "title+abstract_embedding_9": 0.06811464, "title+abstract_embedding_10": 0.11259273, "title+abstract_embedding_11": -0.5118729, "title+abstract_embedding_12": 0.19961599, "title+abstract_embedding_13": -0.18477887, "title+abstract_embedding_14": -0.12327002, "title+abstract_embedding_15": -0.006408682, "title+abstract_embedding_16": 0.18667716, "title+abstract_embedding_17": 0.16522211, "title+abstract_embedding_18": -0.14187801, 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"title+abstract_embedding_64": -0.2194725, "title+abstract_embedding_65": -0.22029576, "title+abstract_embedding_66": -0.004048929, "title+abstract_embedding_67": -0.1632967, "title+abstract_embedding_68": -0.22715393, "title+abstract_embedding_69": -0.04106777, "title+abstract_embedding_70": 0.3635019, "title+abstract_embedding_71": -0.02529563, "title+abstract_embedding_72": 0.15913817, "title+abstract_embedding_73": -0.11778973, "title+abstract_embedding_74": 0.03640241, "title+abstract_embedding_75": 0.15938248, "title+abstract_embedding_76": 0.23927575, "title+abstract_embedding_77": 0.013733089, "title+abstract_embedding_78": 0.08484577, "title+abstract_embedding_79": 0.002495617, "title+abstract_embedding_80": 0.016775597, "title+abstract_embedding_81": 0.14363614, "title+abstract_embedding_82": 0.03338769, "title+abstract_embedding_83": 0.059510734, "title+abstract_embedding_84": -0.07816939, "title+abstract_embedding_85": -0.016745975, "title+abstract_embedding_86": -0.083052434, "title+abstract_embedding_87": 0.033752803, "title+abstract_embedding_88": 0.068615094, "title+abstract_embedding_89": 0.04388259, "title+abstract_embedding_90": -0.18741497, "title+abstract_embedding_91": -0.099563666, "title+abstract_embedding_92": -0.006480284, "title+abstract_embedding_93": -0.04311371, "title+abstract_embedding_94": -0.024658673, "title+abstract_embedding_95": 0.11399602, "title+abstract_embedding_96": 0.0220607, "title+abstract_embedding_97": 0.10054782, "title+abstract_embedding_98": -0.09135403, "title+abstract_embedding_99": 0.071001835, "title+abstract_embedding_100": 0.059009593, "title+abstract_embedding_101": -0.033169582, "title+abstract_embedding_102": -0.16591617, "title+abstract_embedding_103": 0.111094475, "title+abstract_embedding_104": 0.21577398, "title+abstract_embedding_105": -0.30058533, "title+abstract_embedding_106": -0.1128701, "title+abstract_embedding_107": 0.065920055, "title+abstract_embedding_108": 0.07428914, "title+abstract_embedding_109": -0.061891496, "title+abstract_embedding_110": -0.13129638, "title+abstract_embedding_111": 0.21052963, "title+abstract_embedding_112": 0.05758339, "title+abstract_embedding_113": 0.049594104, "title+abstract_embedding_114": -0.06174983, "title+abstract_embedding_115": 0.01033628, "title+abstract_embedding_116": -0.046815664, "title+abstract_embedding_117": 0.07724678, "title+abstract_embedding_118": 0.07399292, "title+abstract_embedding_119": -0.067395285, "title+abstract_embedding_120": 0.04301958, "title+abstract_embedding_121": -0.03213992, "title+abstract_embedding_122": -0.0363276, "title+abstract_embedding_123": -0.094558716, "title+abstract_embedding_124": -0.03550697, "title+abstract_embedding_125": 0.25167012, "title+abstract_embedding_126": 0.027572215, "title+abstract_embedding_127": -0.1355525, "label": 3, "label-multi": "3" }, { "paper_new_id": 184, "id": "j_e91fa4f3fac3d8c66bd82de7420cb6e0", "title+abstract": "Efficient electrocatalytic reduction of CO2 to HCOOH by bimetallic In-Cu nanoparticles with controlled growth facet;Abstract The electrochemical reduction of CO2 to formic acid (HCOOH) by Indium (In)-based materials have been considered an effective way to solve the energy crisis. Unfortunately, In-based materials face a low selectivity for HCOOH in CO2 reduction reaction (CO2RR) systems. Here, we have successfully prepared bimetallic InxCuy (x, y are the molar ratio) nanoparticles (NPs) electrocatalysts. For the first time, we adjust the growth direction of the electrocatalysts crystal facets by changing the In/Cu ratio in the electrocatalysts structure, so that the Faraday efficiency of HCOOH by In-based materials are raised to a new level (90 % at -1.2 V vs. RHE). Indeed, DFT calculations further showed that the In (101) facet of in InxCuy NPs stabilizes the *OCHO intermediate more effectively, thereby reducing the potential for CO2 to HCOOH. The insights gained from this work can lay the foundation for designing efficient electrocatalysts for the reduction of CO2 to HCOOH.", "title+abstract_embedding_0": -0.48072922, "title+abstract_embedding_1": -0.6509559, "title+abstract_embedding_2": 0.38371003, "title+abstract_embedding_3": -0.3690437, "title+abstract_embedding_4": 0.41983014, "title+abstract_embedding_5": 0.061131418, "title+abstract_embedding_6": -0.16860351, "title+abstract_embedding_7": -0.19361785, "title+abstract_embedding_8": -0.03193406, "title+abstract_embedding_9": 0.15011525, "title+abstract_embedding_10": -0.27950138, "title+abstract_embedding_11": -0.11189136, "title+abstract_embedding_12": 0.26735812, "title+abstract_embedding_13": 0.17038116, "title+abstract_embedding_14": -0.13333163, "title+abstract_embedding_15": -0.40247986, "title+abstract_embedding_16": 0.19427025, "title+abstract_embedding_17": -0.05457215, "title+abstract_embedding_18": 0.020926818, "title+abstract_embedding_19": -0.011889799, "title+abstract_embedding_20": 0.39017463, "title+abstract_embedding_21": 0.30077735, "title+abstract_embedding_22": -0.41028652, "title+abstract_embedding_23": 0.36236036, "title+abstract_embedding_24": 0.01883623, "title+abstract_embedding_25": 0.2813465, "title+abstract_embedding_26": 0.05705183, "title+abstract_embedding_27": -0.11297159, "title+abstract_embedding_28": 0.2726767, "title+abstract_embedding_29": -0.14483277, "title+abstract_embedding_30": 0.3556529, "title+abstract_embedding_31": -0.067416094, "title+abstract_embedding_32": -0.013098232, "title+abstract_embedding_33": 0.24658419, "title+abstract_embedding_34": -0.16335645, "title+abstract_embedding_35": 0.18687063, "title+abstract_embedding_36": 0.06499526, "title+abstract_embedding_37": -0.012781024, "title+abstract_embedding_38": -0.068788886, "title+abstract_embedding_39": -0.027567875, "title+abstract_embedding_40": 0.17603031, "title+abstract_embedding_41": -0.041607756, "title+abstract_embedding_42": 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"title+abstract_embedding_65": -0.060400717, "title+abstract_embedding_66": 0.20625438, "title+abstract_embedding_67": 0.12273908, "title+abstract_embedding_68": -0.07491672, "title+abstract_embedding_69": -0.011567913, "title+abstract_embedding_70": 0.056393642, "title+abstract_embedding_71": -0.2414317, "title+abstract_embedding_72": -0.08094631, "title+abstract_embedding_73": -0.024960034, "title+abstract_embedding_74": 0.10595563, "title+abstract_embedding_75": 0.23664916, "title+abstract_embedding_76": 0.28405005, "title+abstract_embedding_77": 0.16648221, "title+abstract_embedding_78": -0.049523436, "title+abstract_embedding_79": -0.13018045, "title+abstract_embedding_80": -0.050264552, "title+abstract_embedding_81": 0.13389345, "title+abstract_embedding_82": -0.032696635, "title+abstract_embedding_83": -0.04144027, "title+abstract_embedding_84": 0.027883336, "title+abstract_embedding_85": 0.032146286, "title+abstract_embedding_86": -0.06786349, "title+abstract_embedding_87": -0.09764704, "title+abstract_embedding_88": 0.072865695, "title+abstract_embedding_89": -0.1593557, "title+abstract_embedding_90": -0.02483777, "title+abstract_embedding_91": 0.062309306, "title+abstract_embedding_92": 0.09742513, "title+abstract_embedding_93": -0.08106704, "title+abstract_embedding_94": -0.05634909, "title+abstract_embedding_95": -0.00060143, "title+abstract_embedding_96": 0.007087447, "title+abstract_embedding_97": 0.0673558, "title+abstract_embedding_98": 0.0435258, "title+abstract_embedding_99": 0.08674071, "title+abstract_embedding_100": -0.003018461, "title+abstract_embedding_101": 0.14992179, "title+abstract_embedding_102": -0.052837327, "title+abstract_embedding_103": -0.030388445, "title+abstract_embedding_104": 0.06571967, "title+abstract_embedding_105": 0.061950292, "title+abstract_embedding_106": 0.03561066, "title+abstract_embedding_107": 0.06039439, "title+abstract_embedding_108": 0.019652903, "title+abstract_embedding_109": -0.067341715, "title+abstract_embedding_110": -0.00086996, "title+abstract_embedding_111": -0.2910671, "title+abstract_embedding_112": -0.036450878, "title+abstract_embedding_113": -0.07088953, "title+abstract_embedding_114": 0.000985369, "title+abstract_embedding_115": -0.019441769, "title+abstract_embedding_116": 0.06603219, "title+abstract_embedding_117": -0.063224286, "title+abstract_embedding_118": -0.28085157, "title+abstract_embedding_119": 0.025053635, "title+abstract_embedding_120": -0.10593721, "title+abstract_embedding_121": -0.22759867, "title+abstract_embedding_122": -0.041758448, "title+abstract_embedding_123": -0.040920366, "title+abstract_embedding_124": -0.047075666, "title+abstract_embedding_125": -0.030465104, "title+abstract_embedding_126": -0.04058836, "title+abstract_embedding_127": 0.107470036, "label": 3, "label-multi": "0;3" }, { "paper_new_id": 185, "id": "j_ec307970e261e26b7ec96879f39ead16", "title+abstract": "Development of enhanced materials for direct-methanol fuel cell by combinatorial method and nanoscience;Abstract In this review we selectively summarize recent progress, in the development of the direct-methanol fuel cell (DMFC). The paper is mainly focused on research of electrocatalysts and electrolyte membranes, which are the important materials in DMFC that is a power generator to convert a chemical energy to electrical energy. However, in spite of a huge amount of work on these materials, there are still many obstacles that should be overcome for commercialization of DMFC. Here, we report the approaches of combinatorial method and nanoscience for developing electrocatalsyts and electrolyte membranes.", "title+abstract_embedding_0": -1.6044023, "title+abstract_embedding_1": -1.0005322, "title+abstract_embedding_2": 0.051106364, "title+abstract_embedding_3": 0.52625716, "title+abstract_embedding_4": -0.31016958, "title+abstract_embedding_5": 0.6666381, "title+abstract_embedding_6": -0.33449402, "title+abstract_embedding_7": -0.13293651, "title+abstract_embedding_8": 0.15893632, "title+abstract_embedding_9": 0.17068416, "title+abstract_embedding_10": 0.37023035, "title+abstract_embedding_11": 0.09397432, "title+abstract_embedding_12": -0.22721648, "title+abstract_embedding_13": -0.26368102, "title+abstract_embedding_14": -0.30846122, "title+abstract_embedding_15": 0.20490293, "title+abstract_embedding_16": -0.033315703, "title+abstract_embedding_17": -0.71518683, "title+abstract_embedding_18": 0.011694834, "title+abstract_embedding_19": -0.074472755, "title+abstract_embedding_20": -0.5560085, "title+abstract_embedding_21": -0.08576137, "title+abstract_embedding_22": -0.22877325, "title+abstract_embedding_23": -0.114411175, "title+abstract_embedding_24": 0.3040631, "title+abstract_embedding_25": -0.44606316, "title+abstract_embedding_26": 0.1941131, "title+abstract_embedding_27": 0.47483435, "title+abstract_embedding_28": 0.30350918, "title+abstract_embedding_29": -0.27681714, "title+abstract_embedding_30": 0.040420204, "title+abstract_embedding_31": -0.06600288, "title+abstract_embedding_32": -0.15077132, "title+abstract_embedding_33": -0.011054903, "title+abstract_embedding_34": -0.06598616, "title+abstract_embedding_35": -0.15677208, "title+abstract_embedding_36": 0.055918425, "title+abstract_embedding_37": 0.04788448, "title+abstract_embedding_38": -0.7220659, "title+abstract_embedding_39": 0.295173, "title+abstract_embedding_40": -0.13610551, "title+abstract_embedding_41": 0.18688717, "title+abstract_embedding_42": -0.010477185, "title+abstract_embedding_43": 0.21146242, "title+abstract_embedding_44": -0.010668859, "title+abstract_embedding_45": 0.4543944, "title+abstract_embedding_46": -0.045797527, "title+abstract_embedding_47": -0.1748657, "title+abstract_embedding_48": 0.3844918, "title+abstract_embedding_49": -0.015964039, "title+abstract_embedding_50": 0.08493499, "title+abstract_embedding_51": 0.12160489, "title+abstract_embedding_52": -0.08761763, "title+abstract_embedding_53": 0.15084298, "title+abstract_embedding_54": 0.3437513, "title+abstract_embedding_55": 0.22081167, "title+abstract_embedding_56": -0.08914963, "title+abstract_embedding_57": 0.30956554, "title+abstract_embedding_58": 0.20365487, "title+abstract_embedding_59": -0.16170631, "title+abstract_embedding_60": 0.21070683, "title+abstract_embedding_61": -0.014144123, "title+abstract_embedding_62": -0.08708565, "title+abstract_embedding_63": 0.088063076, "title+abstract_embedding_64": 0.16213141, "title+abstract_embedding_65": 0.0432875, "title+abstract_embedding_66": -0.29152644, "title+abstract_embedding_67": 0.12284097, "title+abstract_embedding_68": -0.013638064, "title+abstract_embedding_69": -0.061522543, "title+abstract_embedding_70": 0.054860145, "title+abstract_embedding_71": 0.111221954, "title+abstract_embedding_72": 0.2692974, "title+abstract_embedding_73": -0.16824163, "title+abstract_embedding_74": -0.33305353, "title+abstract_embedding_75": -0.06617154, "title+abstract_embedding_76": 0.16725153, "title+abstract_embedding_77": -0.051393077, "title+abstract_embedding_78": -0.03282728, "title+abstract_embedding_79": -0.13019675, "title+abstract_embedding_80": 0.15196756, "title+abstract_embedding_81": -0.09172765, "title+abstract_embedding_82": -0.26909018, "title+abstract_embedding_83": -0.18362041, "title+abstract_embedding_84": -0.15530895, "title+abstract_embedding_85": -0.013801897, "title+abstract_embedding_86": -0.059613876, "title+abstract_embedding_87": -0.014275916, "title+abstract_embedding_88": 0.25067565, "title+abstract_embedding_89": 0.03209784, "title+abstract_embedding_90": 0.24343738, "title+abstract_embedding_91": -0.2659496, "title+abstract_embedding_92": 0.11882307, "title+abstract_embedding_93": -0.09157849, "title+abstract_embedding_94": 0.5148901, "title+abstract_embedding_95": 0.016438114, "title+abstract_embedding_96": -0.27123535, "title+abstract_embedding_97": -0.072847456, "title+abstract_embedding_98": 0.11734867, "title+abstract_embedding_99": -0.13633734, "title+abstract_embedding_100": 0.13626924, "title+abstract_embedding_101": -0.013756093, "title+abstract_embedding_102": 0.07286987, "title+abstract_embedding_103": 0.08715449, "title+abstract_embedding_104": 0.005821616, "title+abstract_embedding_105": -0.12241171, "title+abstract_embedding_106": 0.051053047, "title+abstract_embedding_107": -0.15303376, "title+abstract_embedding_108": 0.11015029, "title+abstract_embedding_109": 0.08306594, "title+abstract_embedding_110": 0.043514073, "title+abstract_embedding_111": -0.028831925, "title+abstract_embedding_112": -0.12217419, "title+abstract_embedding_113": -0.009479716, "title+abstract_embedding_114": 0.13171205, "title+abstract_embedding_115": 0.11837724, "title+abstract_embedding_116": 0.05293478, "title+abstract_embedding_117": 0.15438634, "title+abstract_embedding_118": 0.019825172, "title+abstract_embedding_119": -0.100384384, "title+abstract_embedding_120": -0.086108014, "title+abstract_embedding_121": 0.27967328, "title+abstract_embedding_122": -0.0086568, "title+abstract_embedding_123": 0.09597664, "title+abstract_embedding_124": -0.04150302, "title+abstract_embedding_125": -0.03650625, "title+abstract_embedding_126": -0.02851871, "title+abstract_embedding_127": 0.088297784, "label": 3, "label-multi": "0;3" }, { "paper_new_id": 186, "id": "j_ecd9006b64467bc255e0b93e5c646bba", "title+abstract": "Synthesis and photocatalytic activity of Mn-doped TiO2 nanostructured powders under UV and visible light;Abstract A straight forward, simple and inexpensive process has been developed by sol¡§Cgel method for the synthesis of manganese (Mn) doped and undoped TiO2 photocatalysts. X-ray powder diffractometry (XRD), scanning electron microscopy (SEM) and transmission electron microscopy (TEM) revealed the presence of structural nanoparticles with an average nanocrystalline size of about 20?nm. FT-IR/vis adsorption has shown enhanced sub-band-gap absorption as a function of Mn concentration. The photocatalytic activity of these materials was evaluated by the degradation of a basic Methylene Blue (MB) as organic contaminant. Mn-doped TiO2 powder with molar ratio 0.1:100 was mixed with calcareous filler (5% and 10% respectively) and the photocatalytic activity was evaluated by the degradation of inorganic pollutants such as NOx under UV and visible light.", "title+abstract_embedding_0": 0.48217607, "title+abstract_embedding_1": 0.89420104, "title+abstract_embedding_2": -0.8004148, "title+abstract_embedding_3": 0.4815042, "title+abstract_embedding_4": 0.12474829, "title+abstract_embedding_5": -0.07067084, "title+abstract_embedding_6": -0.10932797, "title+abstract_embedding_7": 0.15444905, "title+abstract_embedding_8": 0.05241116, "title+abstract_embedding_9": 0.12905854, "title+abstract_embedding_10": -0.08442527, "title+abstract_embedding_11": -0.15310837, "title+abstract_embedding_12": 0.16904977, "title+abstract_embedding_13": -0.15054956, "title+abstract_embedding_14": 0.2222273, "title+abstract_embedding_15": -0.16685058, "title+abstract_embedding_16": 0.15150881, "title+abstract_embedding_17": 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"title+abstract_embedding_108": 0.2533486, "title+abstract_embedding_109": -0.042928725, "title+abstract_embedding_110": 0.022809982, "title+abstract_embedding_111": 0.019418266, "title+abstract_embedding_112": -0.09985499, "title+abstract_embedding_113": -0.015015036, "title+abstract_embedding_114": 0.11914772, "title+abstract_embedding_115": 0.02105578, "title+abstract_embedding_116": 0.008129172, "title+abstract_embedding_117": -0.090428576, "title+abstract_embedding_118": 0.020450886, "title+abstract_embedding_119": -0.103383675, "title+abstract_embedding_120": 0.023637913, "title+abstract_embedding_121": 0.046384502, "title+abstract_embedding_122": -0.00435251, "title+abstract_embedding_123": 0.027135246, "title+abstract_embedding_124": -0.045965098, "title+abstract_embedding_125": 0.023925755, "title+abstract_embedding_126": 0.050063662, "title+abstract_embedding_127": 0.072900504, "label": 3, "label-multi": "0;3" }, { "paper_new_id": 187, "id": "j_ee22e0765cb0027f579967c7965d1981", "title+abstract": "Applications of MXene (Ti3C2Tx) in photocatalysis: a review;MXenes are two-dimensional nanomaterials, which can be constructed from different elements.
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"title+abstract_embedding_114": 0.12663895, "title+abstract_embedding_115": 0.1066809, "title+abstract_embedding_116": 0.011488434, "title+abstract_embedding_117": 0.043791156, "title+abstract_embedding_118": 0.055755716, "title+abstract_embedding_119": -0.34046394, "title+abstract_embedding_120": -0.19203217, "title+abstract_embedding_121": -0.23946565, "title+abstract_embedding_122": 0.16658947, "title+abstract_embedding_123": 0.013454124, "title+abstract_embedding_124": 0.07251231, "title+abstract_embedding_125": -0.21421215, "title+abstract_embedding_126": 0.17805515, "title+abstract_embedding_127": -0.05653909, "label": 1, "label-multi": "1" }, { "paper_new_id": 188, "id": "j_effad726041782f2013a464a1f8af529", "title+abstract": "Photocatalytic comparison of Cu- and Ag-doped TiO2/GF for bioaerosol disinfection under visible light;Abstract Photocatalysts, TiO 2 /glass fiber (TiO 2 /GF), Cu-doped TiO 2 /glass fiber (Cu¡§CTiO 2 /GF) and Ag-doped TiO 2 /glass fiber (Ag¡§CTiO 2 /GF), were synthesized by a sol¡§Cgel method. They were then used to disinfect Escherichia coli ( E. coli ) and Staphylococcus aureus ( S. aureus ) in bioaerosols under visible light irradiation. TiO 2 /GF did not show any significant disinfection effect. Both Cu and Ag acted as intermediate agents to enhance separation efficiency of electron¡§Chole pairs of TiO 2 , leading to improved photocatalytic activity of Cu¡§CTiO 2 /GF and Ag¡§CTiO 2 /GF under visible light. Cu in Cu¡§CTiO 2 /GF acted as a defective agent, increasing the internal quantum efficiency of TiO 2 , while Ag in Ag¡§CTiO 2 /GF acted as a sensitive agent, enhancing the transfer efficiency of the electrons generated. The highest disinfection efficiencies of E. coli and S. aureus by Cu¡§CTiO 2 /GF were 84.85% and 65.21%, respectively. The highest disinfection efficiencies of E. coli and S. aureus by Ag¡§CTiO 2 /GF were 94.46% and 73.12%, respectively. Among three humidity conditions ¡§C 40?¨¤5% (dry), 60?¨¤5% (moderate), and 80?¨¤5% (humid) ¡§C the moderate humidity condition showed the highest disinfection efficiency for both E. coli and S. aureus . This study also showed that a Gram-negative bacterium ( E. coli ) were more readily disinfected by the photocatalysts than a Gram-positive bacterium ( S. aureus ).", "title+abstract_embedding_0": 0.83126366, "title+abstract_embedding_1": 0.53888685, "title+abstract_embedding_2": 0.65079886, "title+abstract_embedding_3": 0.27432895, "title+abstract_embedding_4": -0.18780172, "title+abstract_embedding_5": 0.018159091, "title+abstract_embedding_6": 0.02264756, "title+abstract_embedding_7": 0.17328355, "title+abstract_embedding_8": -0.40294626, "title+abstract_embedding_9": -0.2403943, "title+abstract_embedding_10": -0.25742903, "title+abstract_embedding_11": 0.19315204, "title+abstract_embedding_12": 0.12152706, "title+abstract_embedding_13": 0.29325238, "title+abstract_embedding_14": -0.6494944, "title+abstract_embedding_15": 0.5631955, "title+abstract_embedding_16": -0.38952816, "title+abstract_embedding_17": -0.051047787, "title+abstract_embedding_18": -0.23564929, 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"title+abstract_embedding_110": 0.035993367, "title+abstract_embedding_111": -0.04079487, "title+abstract_embedding_112": -0.19666578, "title+abstract_embedding_113": 0.040778384, "title+abstract_embedding_114": 0.040717646, "title+abstract_embedding_115": 0.06973006, "title+abstract_embedding_116": 0.07219451, "title+abstract_embedding_117": 0.03599213, "title+abstract_embedding_118": -0.11412447, "title+abstract_embedding_119": -0.037203014, "title+abstract_embedding_120": 0.05271742, "title+abstract_embedding_121": 0.037570603, "title+abstract_embedding_122": 0.013768405, "title+abstract_embedding_123": 0.02558627, "title+abstract_embedding_124": -0.010958508, "title+abstract_embedding_125": -0.08318392, "title+abstract_embedding_126": 0.010968324, "title+abstract_embedding_127": 0.08523452, "label": 3, "label-multi": "3" }, { "paper_new_id": 189, "id": "j_f0abc6f08490944a1273e4990b440475", "title+abstract": "Efficient Photocatalytic Oxidation of Cycloalkenes by Dihydroxo(tetraphenylporphyrinato)antimony Supported on Silica Gel under Visible Light Irradiation;In order to develop a photocatalyst operating under visible light irradiation, silica gel-supported dihydroxo(tetraphenylporphyrinato)antimony (V) complex, SbTPP(OH) 2 ] + /SiO 2 . was prepared. The photocatalytic oxidationof cycloalkenes with oxygen molecule was performed on [SbTPP(OH) 2 ] /SiO 2 particles under irradiation of fluorescent light. The photocatalytic oxidation of cycloalkenes gave the corresponding cis-1,2-epoxycycloalkane, 2-cycloalkene-1-ol, and trans-1,2-cycloalkanediol.", "title+abstract_embedding_0": 0.001917362, "title+abstract_embedding_1": 1.5473951, "title+abstract_embedding_2": 0.61938775, "title+abstract_embedding_3": -0.335217, "title+abstract_embedding_4": -0.033417165, "title+abstract_embedding_5": 0.106731474, "title+abstract_embedding_6": -0.6166035, "title+abstract_embedding_7": 0.55612874, "title+abstract_embedding_8": -0.031243332, "title+abstract_embedding_9": -0.19848669, "title+abstract_embedding_10": 0.38897836, "title+abstract_embedding_11": 0.28387713, "title+abstract_embedding_12": -0.06133026, "title+abstract_embedding_13": -0.08180355, "title+abstract_embedding_14": -0.16477054, "title+abstract_embedding_15": -0.37374997, "title+abstract_embedding_16": -0.31479573, "title+abstract_embedding_17": -0.007012516, "title+abstract_embedding_18": 0.30759686, "title+abstract_embedding_19": 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"title+abstract_embedding_110": 0.023570955, "title+abstract_embedding_111": -0.20135829, "title+abstract_embedding_112": 0.083431125, "title+abstract_embedding_113": 0.13881844, "title+abstract_embedding_114": -0.07624839, "title+abstract_embedding_115": -0.08216592, "title+abstract_embedding_116": 0.06109251, "title+abstract_embedding_117": -0.009955138, "title+abstract_embedding_118": -0.059347413, "title+abstract_embedding_119": 0.09484154, "title+abstract_embedding_120": 0.15023062, "title+abstract_embedding_121": 0.25490564, "title+abstract_embedding_122": 0.16177878, "title+abstract_embedding_123": 0.10167756, "title+abstract_embedding_124": 0.07590893, "title+abstract_embedding_125": -0.06458061, "title+abstract_embedding_126": 0.10469854, "title+abstract_embedding_127": 0.06981176, "label": 3, "label-multi": "3" }, { "paper_new_id": 190, "id": "j_f189ee15907522a758fb51ac37c58751", "title+abstract": "Enhanced photocatalytic activity of bismuth-doped TiO2 nanotubes under direct sunlight irradiation for degradation of Rhodamine B dye;Bismuth-doped TiO2 nanotubes (Bi-TNT) were successfully synthesized by combination of sol¡§Cgel and hydrothermal methods. The synthesized photocatalyst was efficiently used for degradation of rhodamine B (RhB) dye under direct sunlight irradiation. Subsequent characterization of synthesized photocatalysts was carried out using PXRD, SEM, TEM, EDX, FT-IR, Raman, N2 adsorption, TPD-NH3, UV¡§CVis DRS, XRF and ICP techniques. The surface area of the TiO2 nanoparticles increased after tubular structure formation (TiO2 nanoparticles?a114.21?m2/g, TiO2 nanotube?a191.93?m2/g). The degradation studies revealed that initial rate of photocatalytic degradation of RhB dye using Bi-TNT was 5.56, 4.16, 1.30 and 2.38 times higher as compared to TNP, Bi-TNP, TNT and Degussa P-25 TiO2 (P-25), respectively, under direct sunlight irradiation. The enhanced photocatalytic activity of Bi-TNT may be due to the increase in the surface area and Bi doping, which leads to effective separation of photogenerated carriers. The degradation was confirmed by chemical oxygen demand, total organic carbon and total inorganic carbon analysis of the degraded dye solutions. The probable degradation mechanism of RhB dye has also been proposed using liquid chromatography-mass spectrometry analysis of degraded samples.", "title+abstract_embedding_0": 0.9432639, "title+abstract_embedding_1": 0.89578855, "title+abstract_embedding_2": 0.15806058, "title+abstract_embedding_3": 0.19010139, "title+abstract_embedding_4": 0.4088512, "title+abstract_embedding_5": -0.05503732, "title+abstract_embedding_6": -0.47117028, "title+abstract_embedding_7": 0.052073587, "title+abstract_embedding_8": -0.07392689, "title+abstract_embedding_9": -0.28335226, "title+abstract_embedding_10": 0.10509217, "title+abstract_embedding_11": -0.12106089, "title+abstract_embedding_12": 0.23453349, "title+abstract_embedding_13": -0.55783474, "title+abstract_embedding_14": -0.10160352, "title+abstract_embedding_15": -0.34689817, "title+abstract_embedding_16": -0.048596114, "title+abstract_embedding_17": 0.041803837, "title+abstract_embedding_18": -0.09767661, "title+abstract_embedding_19": 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"title+abstract_embedding_110": -0.056445703, "title+abstract_embedding_111": -0.06451815, "title+abstract_embedding_112": -0.041245386, "title+abstract_embedding_113": -0.08842541, "title+abstract_embedding_114": 0.089485645, "title+abstract_embedding_115": 0.151059, "title+abstract_embedding_116": 0.022242017, "title+abstract_embedding_117": -0.07848033, "title+abstract_embedding_118": -0.11653227, "title+abstract_embedding_119": -0.013126447, "title+abstract_embedding_120": -0.008755375, "title+abstract_embedding_121": 0.10911425, "title+abstract_embedding_122": -0.017460793, "title+abstract_embedding_123": 0.022286363, "title+abstract_embedding_124": -0.02145242, "title+abstract_embedding_125": 0.053774036, "title+abstract_embedding_126": 0.008152545, "title+abstract_embedding_127": 0.060910456, "label": 3, "label-multi": "1;15;3" }, { "paper_new_id": 191, "id": "j_f309b6c166c0e99365343404720f3459", "title+abstract": "In Situ Electrodeposited Gold Nanoparticles on Polyaniline-Modified Electrode Surface for the Detection of Dopamine in Presence of Ascorbic Acid and Uric Acid;In this study, in situ electrodeposition of gold nanoparticles (AuNPs) over polyaniline (PANI)-modified glassy carbon electrode (GCE) surface using linear sweep voltammetry (LSV) has been found to be more effective than cyclic voltammetry (CV). LSV prevents stripping of the Au atoms from the electrode surface, thus leading to an efficient loading of AuNPs on the PANI matrix. The reduction of Au over PANI-modified GCE occurs at 0.34 V and the amount of Au loaded using LSV for 15 linear sweep cycles is 54.75 ?¨¢ 10?9 g. Various techniques are employed to characterize the modified electrode surface. Fourier transform infrared spectroscopic studies show that the electroreduction of Au increases the quinoid moieties in PANI, and the X-ray diffraction data reveals the average crystallite size of AuNPs as 65 nm. The field emission scanning electron microscopy and atomic force microscopy analysis indicate the dispersion of spherical AuNPs over the PANI matrix. The electrochemical studies show enhanced electrocatalytic activity of the modified electrode surface at neutral pH, suitable for sensing biomolecule, dopamine (DA) amidst the interferences, ascorbic acid (AA), and uric acid (UA). The oxidation of DA reported to occur in the range of 0.270 V to 0.361 V for PANI-AuNPs based electrodes at neutral pH is lowered to 0.168 V at the modified electrode surface prepared electrochemically in the present study. The peak-to-peak separation for DA-AA and DA-UA is 108 mV and 345 mV, respectively, with the working linear range of 20¡§C100 |¨¬M and a detection limit of 16 |¨¬M for DA. Such enhanced electrocatalytic response is attributed to a synergistic interaction between the PANI film and electrodeposited AuNPs.", "title+abstract_embedding_0": 0.66483295, "title+abstract_embedding_1": -1.1307213, "title+abstract_embedding_2": 0.05440259, "title+abstract_embedding_3": 0.2600876, "title+abstract_embedding_4": -0.21710163, "title+abstract_embedding_5": -0.65854096, "title+abstract_embedding_6": 0.07546097, "title+abstract_embedding_7": 0.31460655, "title+abstract_embedding_8": -0.300954, "title+abstract_embedding_9": -0.5797596, "title+abstract_embedding_10": -0.23527738, "title+abstract_embedding_11": 0.34974417, "title+abstract_embedding_12": 0.2344127, "title+abstract_embedding_13": 0.3119973, "title+abstract_embedding_14": 0.07955861, "title+abstract_embedding_15": 0.032786984, "title+abstract_embedding_16": 0.24465603, "title+abstract_embedding_17": -0.091824844, "title+abstract_embedding_18": 0.2659732, "title+abstract_embedding_19": -0.094906375, 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Aminobenzenes Having Reducible Groups by a Titanium(IV) Oxide Photocatalyst under Gas- and Metal-Free Conditions.;The title reaction is performed in the presence of oxalic acid as a hole scavenger without the use of a precious metal or a reducing gas.", "title+abstract_embedding_0": -1.7313447, "title+abstract_embedding_1": 0.61248267, "title+abstract_embedding_2": 0.45582086, "title+abstract_embedding_3": 0.15642017, "title+abstract_embedding_4": -0.40579814, "title+abstract_embedding_5": 0.070797205, "title+abstract_embedding_6": -0.71077883, "title+abstract_embedding_7": 0.9429264, "title+abstract_embedding_8": 0.27897707, "title+abstract_embedding_9": 0.15671146, "title+abstract_embedding_10": 0.21548486, "title+abstract_embedding_11": -1.0911292, "title+abstract_embedding_12": 0.6504361, "title+abstract_embedding_13": 0.5439102, "title+abstract_embedding_14": -0.11447509, "title+abstract_embedding_15": -0.49736863, "title+abstract_embedding_16": -0.017209172, 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"j_f671c425bbb320061be7b5f9661e26e7", "title+abstract": "Enhanced electrochemical reactions of 1,4-benzoquinone at nanoporous electrodes;We report that the proton-coupled electron transfer kinetics of 1,4-benzoquinone was significantly enhanced in electrified nanopores in aqueous media. At nanoporous Pt and Au electrodes, the voltammetric behaviour of 1,4-benzoquinone at nanoporous electrodes was clearly distinct from that at flat surfaces. Proton transfer as well as electron transfer kinetics were facilitated in the nanopores by the confinement effect, which indicates all factors originated from the geometric features of nano-scale concave space surrounded by inner walls, suggesting how to utilize nanoporous electrodes for electrocatalysis.", "title+abstract_embedding_0": -1.3722461, "title+abstract_embedding_1": -0.79085755, "title+abstract_embedding_2": -0.3336757, "title+abstract_embedding_3": 0.7418165, "title+abstract_embedding_4": -0.23578298, "title+abstract_embedding_5": 0.049863994, "title+abstract_embedding_6": -0.028739661, "title+abstract_embedding_7": -0.087285295, "title+abstract_embedding_8": -0.45508504, "title+abstract_embedding_9": -0.35918784, "title+abstract_embedding_10": 0.27822638, "title+abstract_embedding_11": -0.005477395, "title+abstract_embedding_12": 0.12529418, "title+abstract_embedding_13": -0.116716795, "title+abstract_embedding_14": -0.14503896, "title+abstract_embedding_15": -0.61195195, 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"title+abstract_embedding_107": -0.010959503, "title+abstract_embedding_108": -0.13495977, "title+abstract_embedding_109": 0.16148262, "title+abstract_embedding_110": -0.19809929, "title+abstract_embedding_111": 0.23469865, "title+abstract_embedding_112": 0.013826773, "title+abstract_embedding_113": 0.23224449, "title+abstract_embedding_114": -0.100095265, "title+abstract_embedding_115": -0.015011601, "title+abstract_embedding_116": -0.21295378, "title+abstract_embedding_117": -0.03882307, "title+abstract_embedding_118": 0.19049545, "title+abstract_embedding_119": 0.072307736, "title+abstract_embedding_120": 0.04251206, "title+abstract_embedding_121": -0.006654028, "title+abstract_embedding_122": -0.053482413, "title+abstract_embedding_123": -0.10879792, "title+abstract_embedding_124": -0.13941443, "title+abstract_embedding_125": 0.11772023, "title+abstract_embedding_126": 0.1854329, "title+abstract_embedding_127": 0.1510707, "label": 3, "label-multi": "2;3" }, { "paper_new_id": 194, "id": "j_f739015d044cf0ae01db539b99b5465d", "title+abstract": "Ultralow-Content Iron-Decorated Ni-MOF-74 Fabricated by a Metala??Organic Framework Surface Reaction for Efficient Electrocatalytic Water Oxidation;Transition-metal-organic frameworks (MOFs) have been regarded as one of the most intriguing electrocatalysts because of its low cost and diversity in functional organic groups and metal centers. Different from the common strategies of tuning the ratio of metal centers in multivariate MOFs, here, ultralow-content Fe2O3 is decorated on the surface of monometallic Ni-MOF-74 based on the fast \"phenol-iron (Fe)\" surface reaction between Fe2+ and the surface hydroxyl group in Ni-MOF-74. Benefiting from this flexible method, the Fe loading can be finely modulated and thus a series of Fe-decorated Ni-MOF-74 with different Fe contents are prepared. The optimized 0.6 wt % Fe2O3@Ni-MOF-74 with the Fe loading of 0.6 wt % only needs the overpotential of 264 mV to deliver 10 mA cm-2, which obviously outperforms Fe-free Ni-MOF-74 (323 mV) and other Fe2O3@Ni-MOF-74 and is even superior to the commercial IrO2 benchmark (300 mV). X-ray photoelectron spectroscopy results disclose that Fe decoration can obviously modulate the electronic structure of Ni center in Ni-MOF-74, thereby resulting in enhanced oxygen evolution reaction activity. This work opens up a new avenue to fabricate excellent MOF-based electrocatalysts for direct utilization in an electrocatalytic process.", "title+abstract_embedding_0": 0.05319071, "title+abstract_embedding_1": -0.74307823, "title+abstract_embedding_2": -0.40546694, "title+abstract_embedding_3": -0.9153019, "title+abstract_embedding_4": 0.33028752, "title+abstract_embedding_5": -0.31205082, "title+abstract_embedding_6": 0.6501652, "title+abstract_embedding_7": 0.124250025, "title+abstract_embedding_8": -0.33291027, "title+abstract_embedding_9": 0.29112655, "title+abstract_embedding_10": -0.104780816, "title+abstract_embedding_11": 0.36196604, "title+abstract_embedding_12": -0.033117205, "title+abstract_embedding_13": 0.3772051, "title+abstract_embedding_14": 0.3401563, "title+abstract_embedding_15": 0.08328361, "title+abstract_embedding_16": -0.22973377, "title+abstract_embedding_17": -0.041795895, "title+abstract_embedding_18": -0.18458715, "title+abstract_embedding_19": -0.10540083, 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"title+abstract_embedding_110": -0.005532563, "title+abstract_embedding_111": -0.006831432, "title+abstract_embedding_112": 0.14327697, "title+abstract_embedding_113": 0.20827162, "title+abstract_embedding_114": -0.046456464, "title+abstract_embedding_115": 0.08466039, "title+abstract_embedding_116": 0.046728, "title+abstract_embedding_117": -0.10733323, "title+abstract_embedding_118": 0.03464262, "title+abstract_embedding_119": 0.09068519, "title+abstract_embedding_120": 0.028124291, "title+abstract_embedding_121": -0.04643783, "title+abstract_embedding_122": -0.027555436, "title+abstract_embedding_123": 0.005035155, "title+abstract_embedding_124": 0.0346535, "title+abstract_embedding_125": -0.003513575, "title+abstract_embedding_126": 0.0914516, "title+abstract_embedding_127": -0.12015517, "label": 106, "label-multi": NaN }, { "paper_new_id": 195, "id": "j_f845d5f643b28b1eb9fff0f8c5843a1b", "title+abstract": "Intramolecular electronic coupling in porous iron cobalt (oxy)phosphide nanoboxes enhances the electrocatalytic activity for oxygen evolution;The effective intramolecular electronic coupling between the Fe and Co atoms
Core¡§Cshell structures can improve the properties of materials due to their special structure and have attracted considerable attention for their applications in many fields.
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"title+abstract_embedding_114": -0.22075264, "title+abstract_embedding_115": 0.13304183, "title+abstract_embedding_116": 0.32483518, "title+abstract_embedding_117": 0.12886262, "title+abstract_embedding_118": -0.05679504, "title+abstract_embedding_119": 0.16069563, "title+abstract_embedding_120": 0.04978234, "title+abstract_embedding_121": -0.11879134, "title+abstract_embedding_122": -0.22569528, "title+abstract_embedding_123": 0.0570456, "title+abstract_embedding_124": -0.06683225, "title+abstract_embedding_125": 0.24350107, "title+abstract_embedding_126": -0.045767218, "title+abstract_embedding_127": 0.19694132, "label": 3, "label-multi": "27;3" }, { "paper_new_id": 198, "id": "j_fc55718cf86799ac5d0637a49cc1f760", "title+abstract": "Novel exfoliated graphitic-C3N4 hybridised ZnBi2O4 (g-C3N4/ZnBi2O4) nanorods for catalytic reduction of 4-Nitrophenol and its antibacterial activity;Abstract Metal-free Graphitic carbon nitride (g-C3N4) nanoparticle was synthesized by an ultrasound-assisted chemical exfoliation method and g-C3N4/ZnBi2O4 nanorods were prepared by the cost-effective hydrothermal technique. As-synthesized nanoparticles were characterized using XRD, FESEM, HRTEM, EDX, UV, PL, BET and XPS. The photocatalytic activity of the g-C3N4/ZnBi2O4 nanocomposite was investigated by treating 4-Nitrophenol at different pH conditions and maximum reduction of 79 % was observed under visible light irradiation. Antibacterial activity of the g-C3N4/ZnBi2O4 nanoparticles were evaluated by disk diffusion method against E.coli and S.aures. The g-C3N4/ZnBi2O4 nanocomposite showed better antibacterial activity towards G? E.coli. With the effect of ZnBi2O4 doping on to the g-C3N4 host structure, the photocatalytic and antimicrobial efficiency has been enhanced.", "title+abstract_embedding_0": 0.85636127, "title+abstract_embedding_1": 0.3332222, "title+abstract_embedding_2": -0.89783204, "title+abstract_embedding_3": -0.36462283, "title+abstract_embedding_4": -0.3393243, "title+abstract_embedding_5": -0.15208524, "title+abstract_embedding_6": -0.74043155, "title+abstract_embedding_7": 0.12116216, "title+abstract_embedding_8": 0.044789754, "title+abstract_embedding_9": 0.067691356, "title+abstract_embedding_10": 0.15514243, "title+abstract_embedding_11": 0.13759813, "title+abstract_embedding_12": -0.39959934, "title+abstract_embedding_13": 0.19548139, "title+abstract_embedding_14": 0.013671905, "title+abstract_embedding_15": -0.15906511, "title+abstract_embedding_16": 0.017773598, "title+abstract_embedding_17": 0.3608605, "title+abstract_embedding_18": 0.101883754, "title+abstract_embedding_19": 0.08970299, 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"title+abstract_embedding_111": 0.04904131, "title+abstract_embedding_112": -0.13458847, "title+abstract_embedding_113": 0.016599745, "title+abstract_embedding_114": -0.16168709, "title+abstract_embedding_115": -0.027174585, "title+abstract_embedding_116": 0.009393621, "title+abstract_embedding_117": 0.12857041, "title+abstract_embedding_118": 0.08035051, "title+abstract_embedding_119": -0.021704799, "title+abstract_embedding_120": 0.041193306, "title+abstract_embedding_121": 0.04443602, "title+abstract_embedding_122": 0.037996083, "title+abstract_embedding_123": -0.004245035, "title+abstract_embedding_124": 0.003688216, "title+abstract_embedding_125": 0.08679344, "title+abstract_embedding_126": -0.054494116, "title+abstract_embedding_127": -0.06781003, "label": 3, "label-multi": "3" }, { "paper_new_id": 199, "id": "j_fca8059d846ff42aaee5f1f7a53576ea", "title+abstract": "Enhanced oxygen evolution and reduction reactions of porous ternary NiCoFe foam electrodes prepared by dynamic hydrogen template deposition;Abstract Electrodeposition at high current densities provides excellent means for the production of deposits with a high surface area. Porous deposits attract great interest due to their wide range of possible applications in electrocatalysis. In addition, an advanced porous electrode should have both, micro and nanoscaled features. We report the synthesis of a multiscale open porous foam of NiCoFe and its excellent electrocatalytic performance. At a current density of 1?A?cm ?2 a 3D dendritic structure with open pores is obtained with pore walls having a morphology that consists of ??cauliflower-like?¡¥ particles containing open multiscaled dendritic structures. Cyclic voltammograms of a smooth NiCoFe electrode are compared with those of the achieved nanodendritic NiCoFe foam electrode. The catalytic activity of the NiCoFe foam is strongly enhanced for both, the cathodic reduction of oxygen and the anodic evolution of oxygen and shows a good reversibility. 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