Unique Charge-density-wave Order and Fluctuation-induced Phonon Softening in the Optimally-doped Trilayer Cuprate Bi_2Sr_2Ca_2Cu_3O_{10+δ}
Abstract
Resonant inelastic x-ray scattering reveals coherent charge-density-wave order and phonon-coupled fluctuations across trilayers in a high-temperature cuprate superconductor.
Charge-density-wave (CDW) order is a ubiquitous feature of cuprate superconductors that competes with superconductivity. However, its behavior remains poorly understood in trilayer compounds, which contain the optimal number of CuO_2 layers for superconductivity. Here, we report Cu L_3- and O K-edge resonant inelastic x-ray scattering (RIXS) measurements of optimally-doped Bi_{2}Sr_{2}Ca_{2}Cu_{3}O_{10+δ} (Bi2223), the trilayer cuprate with the highest superconducting transition temperature (T_c) among Bi-based cuprates. We observe CDW order with a single in-plane wavevector of {bm q}_{CDW} = (0.25, 0), demonstrating that a coherent CDW order is formed across the trilayers. We also resolve CDW fluctuations emanating from the static order, whose profiles differ between the Cu L_3 and O K edges. The phonon softening occurs where these CDW fluctuations interact with the phonon branch, indicating that the RIXS phonon anomaly is driven by the coupling between CDW fluctuations and the phonon branch.
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