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We describe optimized coherent control methods for two-photon transitions in atoms of a ladder-type three-state energy configuration. Our approach is based on the spatial coherent control scheme which utilizes counter-propagating ultrashort laser pulses to produce complex excitation patterns in an extended space. |
Experiments on atoms in intense laser pulses and the corresponding exact ab initio solutions of the time-dependent Schrödinger equation (TDSE) yield photoelectron spectra with low-energy features that are not reproduced by the otherwise successful work horse of strong field laser physics: the "strong field approxim... |
By measuring the transmission of near-resonant light through an atomic vapor confined in a nano-cell we demonstrate a mesoscopic optical response arising from the non-locality induced by the motion of atoms with a phase coherence length larger than the cell thickness. Whereas conventional dispersion theory -- where th... |
The use of Slater-type spinor orbitals in algebraic solution of the Dirac equation is investigated. The one- and two-center integrals constitute the matrix elements arising in generalized eigenvalue equation for one-electron atoms and molecules are evaluated over Slater-type spinor orbitals via ellipsoidal coordinates... |
We report the measurement of absolute excitation frequencies of 87Rb to nS and nD Rydberg states. The Rydberg transition frequencies are obtained by observing electromagnetically induced transparency on a rubidium vapor cell. |
We discuss the results of the calculation of the photoionization with de-excitation of excited He and helium-like ions Li$^{+}$ and B$^{3+}$ at high but non-relativistic photon energies $\omega $. Several lower $^{1}S$ and $^{3}S$ states are considered. |
We demonstrate and characterize a high-flux beam source for cold, slow atoms or molecules. The desired species is vaporized using laser ablation, then cooled by thermalization in a cryogenic cell of buffer gas. |
We investigate the quantum interference between the resonant process of nuclear excitation by electron capture (NEEC) followed by the radiative decay of the excited nucleus, and radiative recombination (RR). In order to derive the interference cross section, a Feshbach projection operator formalism is used. |
We demonstrate a double optical frequency reference (1529 nm and 1560 nm) for the telecom C-band using $^{87}$Rb modulation transfer spectroscopy. The two reference frequencies are defined by the 5S$_{1/2} F=2 \rightarrow $ 5P$_{3/2} F'=3$ two-level and 5S$_{1/2} F=2 \rightarrow $ 5P$_{3/2} F'=3 \rightarrow $ ... |
We experimentally investigate the Bragg reflection of light at one-dimensionally ordered atomic structures by using cold atoms trapped in a laser standing wave. By a fine tuning of the periodicity, we reach the regime of multiple reflection due to the refractive index contrast between layers, yielding an unprecedented... |
The lifetime of Ba$^+$ ions confined in a Paul trap is found, under typical conditions, to be limited by chemical reactions with residual background gas. An integrated ion trap and time-of-flight mass spectrometer are used to analyze the reactions of the trapped Ba$^+$ ions with three common gases in an ultrahigh vacu... |
Transition of an electron from a free to a bound state is critical in determining the qualitative shape of the spectrum in high-order harmonic generation (HHG), and in tomographic imaging of orbitals. We calculate and compare the recombination amplitude, from a continuum state described by a plane wave and an outgoing... |
The angular distribution of the emitted electrons, following the two--photon ionization of the hydrogen--like ions, is studied within the framework of second order perturbation theory \textit{and} the Dirac equation. Using a density matrix approach, we have investigated the effects which arise from the polarization of... |
We investigate the energy levels of heteronuclear alkali metal dimers in levels correlating with the lowest rotational level of the ground electronic state, which are important in efforts to produce ground-state ultracold molecules. We use density-functional theory to calculate nuclear quadrupole and magnetic coupling... |
Local Lorentz Invariance violating (LLIV) and Einstein equivalence principle violating (EEPV) effects in atomic experiments are discussed. The EEPV effects are strongly enhanced in the narrow 7.8 eV transition in 229Th nucleus. |
We present here the results of our relativistic many-body calculations of various properties of the first six low-lying excited states of indium. The calculations were performed using the relativistic coupled-cluster method in the framework of the singles, doubles and partial triples approximation. |
We demonstrate optical sideband spectroscopy of a single $^9$Be$^+$ ion in a cryogenic 5 Tesla Penning trap using two-photon stimulated-Raman transitions between the two Zeeman sublevels of the $1s^{2}2s$ ground state manifold. By applying two complementary coupling schemes, we accurately measure Raman resonances with... |
Engineering a Terahertz (THz) frequency comb spectroscopy at atomic level advances the precisely measurement in spectroscopy and sensing. Current progresses on THz frequency comb rely on difference-frequency generation, optical parametric oscillation, and other methods. |
We explore a technique for decelerating molecules using a static magnetic field and optical pumping. Molecules travel through a spatially varying magnetic field and are repeatedly pumped into a weak-field seeking state as they move towards each strong field region, and into a strong-field seeking state as they move to... |
We derive a quantum master equation for an atom coupled to a heat bath represented by a charged particle many-body environment. In Born-Markov approximation, the influence of the plasma environment on the reduced system is described by the dynamical structure factor. |
For atomic frequency standards in which fluctuations of the local oscillator (LO) frequency are the dominant noise source, we examine the role of the servo algorithm that predicts and corrects these frequency fluctuations. We derive the optimal linear prediction algorithm, showing how to measure the relevant spectral ... |
In recent publications, it has been shown that high-order harmonic generation can be manipulated by employing a time-delayed attosecond pulse train superposed to a strong, near-infrared laser field. It is an open question, however, which is the most adequate way to approximate the attosecond pulse train in a semi-anal... |
We report photoassociative spectroscopy of $^{88}$Sr$_2$ in a magneto-optical trap operating on the ${^1S_0}\to{^3P_1}$ intercombination line at 689 nm. Photoassociative transitions are driven with a laser red-detuned by 600-2400 MHz from the ${^1S_0}\to{^1P_1}$ atomic resonance at 461 nm. |
The kinetics of the OH + CO reaction, fundamental to both atmospheric and combustion chemistry, are complex due to the formation of the HOCO intermediate. Despite extensive studies on this reaction, HOCO has not been observed at thermal reaction conditions. |
We present a theoretical analysis of rf association of Efimov trimers in a 2-component Bose gas with short-range interactions. Using the adiabatic hyperspherical Green's function formalism to solve the quantum 3-body problem, we obtain universal expressions for 3-body rf association rates as a function of the s-wa... |
In the presence of P-violating interactions, the exchange of vector bosons between electrons and nucleons induces parity-nonconserving (PNC) effects in atoms and molecules, while the exchange of vector bosons between nucleons induces anapole moments of nuclei. We perform calculations of such vector-mediated PNC effect... |
In this paper, we have carried out the calculations of the weighted oscillator strengths and the transition probabilities for a few low-lying transitions of boron-like ions: Mg VIII, Si X and S XII which are astrophysically important, particularly, in the atmospheres of the solar corona. We have employed an all-order ... |
We study the time-dependent response of a cold atom cloud illuminated by a laser beam immediately after the light is switched on experimentally and theoretically. We show that cooperative effects, which have been previously investigated in the decay dynamics after the laser is switched off, also give rise to character... |
The techniques of principal and independent component analysis are applied to images of ultracold atoms. As an illustrative example, we present the use of these model-independent methods to rapidly determine the differential phase of a BEC interferometer from large sets of images of interference patterns. |
The interaction between the field emission resonance states and the photodetached electron in an electric field is studied by semiclassical theory. An analytical expression of the photodetachment cross section is derived in the framework. |
Exploiting an approach similar to the R-matrix theory, the diffusion Monte Carlo method is employed to compute phase shifts and threshold cross sections for the elastic scattering of o-positronium off light atoms. Results are obtained for Ps-H and Ps-He as representative cases of open and closed shell targets. |
This work investigates the utility of femtosecond pulse shaping in increasing the efficiency of Raman excitation of molecules in the strong-field interaction regime. We study experimentally and theoretically the effect of pulse shaping on the strength of non-resonant coherent anti-Stokes Raman scattering in iodine vap... |
We study the proton-hydrogen collision in the energy range from 0 to 5 K where the hyperfine structure of the hydrogen atom is important. The proper multichannel treatment of the hyperfine structure is found to be crucial at cold temperatures compared to the elastic approximation used for higher temperatures. |
The existence of cross-over resonances makes saturated-absorption spectra very complicated when external magnetic field B is applied. It is demonstrated for the first time that the use of micrometric-thin cells (MTC, $L\approx40\,\mu$m) allows application of SA for quantitative studies of frequency splittings and shif... |
Bilodeau and Haugan [1], using Infrared laser photodetachment spectroscopy, measured the binding energies (BEs) of the ground state (4Fe9/2) and the excited state (4Fe7/2) of the Os^- ion to be 1.07780(12) eV and 0.553(3) eV, respectively. These values are consistent with those calculated using Relativistic Configurat... |
We present an analysis of systematic sources of uncertainty in a recently proposed scheme for measurement of nuclear-spin-dependent atomic parity violation using two-photon J=0-to-1 transitions driven by collinear photons of the same frequency in the presence of a static magnetic field. Two important sources of uncert... |
Experimental searches for new, "fifth" forces are attracting a lot of attention because they allow to test theoretical extensions to the standard model. Here, we report a new experimental search for possible fifth forces, specifically spin-and-velocity dependent forces, by using a K-Rb-$^{21}$Ne co-magnetomete... |
We determine the transmission of light through a planar atomic array beyond the limit of low light intensity that displays optical bistability in the mean-field regime. We develop a theory describing the intrinsic optical bistability, which is supported purely by resonant dipole-dipole interactions in free space, show... |
Light-pulse atom interferometers based on single-photon transitions are a promising tool for gravitational-wave detection in the mid-frequency band and the search for ultralight dark-matter fields. Here we present a novel measurement scheme that enables their use as freely falling clocks directly measuring relativisti... |
We investigate the effects of impurities, either correlated disorder or a single Gaussian defect, on the collective dipole motion of a Bose-Einstein condensate of $^7$Li in an optical trap. We find that this motion is damped at a rate dependent on the impurity strength, condensate center-of-mass velocity, and interato... |
We address a number of issues regarding solid state electron electric dipole moment (EDM) experiments, focusing on gadolinium iron garnet (abbreviated GdIG, chemical formula Gd$_3$Fe$_5$O$_{12}$) as a possible sample material. GdIG maintains its high magnetic susceptibility down to 4.2 K, which enhances the EDM-induce... |
A new type of decelerator is presented where polar neutral molecules are guided and decelerated using the principle of traveling electric potential wells, such that molecules are confined in stable three-dimensional traps throughout. This new decelerator is superior to the best currently operational decelerator (Schar... |
The autoionization of core-excited Rydberg states is theoretically studied for a broad range of principal and angular-momentum quantum numbers $n$ and $\ell$ in alkaline-earth-metal atoms. We combined two theoretical methods to calculate accurate autoionization rates for $n=10-65$ and $\ell=0-45$ over the 100 orders o... |
Photoassociation of spin-polarized metastable helium to the three lowest rovibrational levels of the J=1, $0_u^+$ state asymptoting to 2$s {}^{3}$S$_{1}+2p {}^{3}$P$_{0}$ is studied using a second-order perturbative treatment of the line shifts valid for low laser intensities, and two variants of a non-perturbative clo... |
Two-photon E1M1 transition rates are evaluated for heliumlike ions with nuclear charges in the range Z = 50-94. The two-photon rates modify previously published lifetimes/transition rates of 2 3P0 states. |
Radiative double electron capture (RDEC), the one-step process occurring in ion-atom collisions, has been investigated for bare fluorine ions colliding with carbon. RDEC is completed when two target electrons are captured to a bound state of a projectile simultaneously with the emission of a single photon. |
We measure spectrally and spatially resolved high-order harmonics generated in argon using chirped multi-cycle laser pulses. Using a stable, high-repetition rate laser we observe detailed interference structures in the far-field. |
Quantum information processing using atomic qubits requires narrow linewidth lasers with long-term stability for high fidelity coherent manipulation of Rydberg states. In this paper, we report on the construction and characterization of three continuous-wave (CW) narrow linewidth lasers stabilized simultaneously to an... |
The synchrotron radiation is commonly known to be completely linearly polarized when observed in the orbital plane of the synchrotron motion. Under actual experimental conditions, however, the degree of polarization of the synchrotron radiation may be lower than the ideal 100%. |
We develop a grid method for multi-channel scattering of atoms in a waveguide with harmonic confinement. This approach is employed to extensively analyze the transverse excitations and deexcitations as well as resonant scattering processes. |
Effective and unrestricted engineering of atom-photon interactions requires precise spatially-resolved control of light beams. The significant potential of such manipulations lies in a set of disciplines ranging from solid state to atomic physics. |
Ab initio QED calculations of the nuclear magnetic shielding constant in helium-like ions are presented. We combine the nonrelativistic QED approach based on an expansion in powers of the fine-structure constant $\alpha$ and the so-called ``all-order'' QED approach which includes all orders in the parameter $Z... |
We demonstrate a simple method to improve the Lewenstein model for the description of high-order harmonic generation (HHG). It is shown that HHG spectra can be expressed as the product of a returning electron wave packet and the photo-recombination cross sections, where the former can be extracted from the Lewenstein ... |
On a dense energy grid reaching up to 75 meV electron collision energy the fragmentation angle and the kinetic energy release of neutral dissociative recombination fragments have been studied in a twin merged beam experiment. The anisotropy described by Legendre polynomials and the extracted rotational state contribut... |
Modifications of photoionization arising from resonant electron-electron correlations between neighbouring atoms in an atomic sample are studied. The sample contains atomic species A and B, with the ionization potential of A being smaller than the energy of a dipole-allowed transition in B. The atoms are subject to an... |
Based on the strong-field approximation, we obtain analytical expressions for the initial momentum at the tunnel exit and instantaneous ionization rate of tunneling ionization in elliptically polarized laser fields with arbitrary ellipticity. The tunneling electron reveals a nonzero offset of the initial momentum at t... |
The Cold-target recoil-ion momentum spectroscopy (COLTRIMS) has been employed to study the single-electron capture processes in collisions of N3+ ions with He atoms at an impact energy of 30 keV. The relative differential cross sections for the capture to different orbitals of N3+ ions are obtained and are compared wi... |
Ion trap systems are a leading platform for large scale quantum computers. Trapped ion qubit crystals are fully-connected and reconfigurable, owing to their long range Coulomb interaction that can be modulated with external optical forces. |
We perform spectroscopic observations of the 698-nm clock transition in $^{87}$Sr confined in an optical lattice using a laser linewidth transfer technique. A narrow-linewidth laser interrogating the clock transition is prepared by transferring the linewidth of a master laser (1064 nm) to that of a slave laser (698 nm... |
We analyze a method of compressing a cloud of cold atoms by dynamic control of a far off resonance optical lattice. We show that by reducing the lattice spacing either continuously or in discrete steps while cooling the atoms with optical molasses large compression factors can be achieved. |
Characterization of the inner-shell decay processes in molecules containing heavy elements is key to understanding x-ray damage of molecules and materials and for medical applications with Auger-electron-emitting radionuclides. The 1s hole states of heavy atoms can be produced by absorption of tunable x-rays and the r... |
Cryogenic buffer gas beams are important sources of cold molecules. In this work we explore the use of a converging-diverging nozzle with a buffer-gas beam. |
Nondipole effects in the atomic dynamic interference are investigated by numerically solving the time-dependent Schrödinger equation~(TDSE) of hydrogen. It is found that the inclusion of nondipole corrections in the TDSE can induce momentum shifts of photoelectrons in the opposite direction of the laser propagation. |
In the recent years there was published some papers in which the photons are represented as electromagnetic solitons [1,2,3]. All particles - solitons - represent some electromagnetic field restricted in a very small volume, length, cross-section and propagate in vacuum with light velocity in one and the same directio... |
We consider the formation of cold ground-state polar molecules in a low vibrational level by laser fields. Starting from a pair of cold colliding atoms of dissimilar species, we propose a strategy consisting of three steps. |
A long-standing problem to account for the electron-positron annihilation in positron Hydrogen scattering above the Positronium formation threshold has been resolved by the use of the three-body Faddeev formalism. The multichannel three-body theory for scattering states in presence of a complex absorbing potential is ... |
We analyze the spatial dynamics of polarized atom vapor and present a mathematical method to eliminate the diffusion effect partially. It is found that the diffusion effect of polarized atoms can be regarded as a low pass filter in spatial frequency domain and fits well with a Butterworth filter. |
We have constructed a magneto-optical trap (MOT) for metastable triplet helium atoms utilizing the 2 3S1 -> 3 3P2 line at 389 nm as the trapping and cooling transition. The far-red-detuned MOT (detuning Delta = -41 MHz) typically contains few times 10^7 atoms at a relatively high (~10^9 cm^-3) density, which is a c... |
Literature mentions only incidentally a sub-Doppler contribution in the excitation spectrum of the backward fluorescence of a dense vapor. This contribution is here investigated on Cs vapor, both on the first resonance line (894 nm) and on the weaker second resonance line (459 nm). |
An all-optical atomic magnetometer is used to detect a proton free-precession signal from a water sample polarized in a 0.7 T field and remotely analyzed in a 4 $\mu T$ field. Nuclear spins are manipulated either by $\pi/2$ pulses or by non-adiabatic rotation. |
We study numerically stabilization against ionization of a fully correlated two-electron model atom in an intense laser pulse. We concentrate on two frequency regimes: very high frequency, where the photon energy exceeds both, the ionization potential of the outer {\em and} the inner electron, and an intermediate freq... |
We have measured the 6s - 7p_{1/2,3/2} transition probabilities in atomic cesium using a direct absorption technique. We use our result plus other previously measured transition rates to derive an accurate value of the vector transition polarizability \beta and, consequently, re-evaluate the weak charge Q_W. |
Based on the geometrical approach to tunnelling by P.D. Hislop and I.M. Sigal [Memoir. AMS 78, No. 399 (1989)], we introduce the concept of a leading tunnelling trajectory. It is then proven that leading tunnelling trajectories for single-active-electron models of molecular tunnelling ionization (i.e., theories where ... |
We report the high resolution photoassociation (PA) spectroscopy of a $^{87}Rb$ Bose-Einstein condensate (BEC) to excited molecular states near the dissociation limit of $5P_{1/2} +5S_{1/2}$ by optical Bragg scattering. Since the detection of optical Bragg scattering in BEC has a high signal-noise ratio, we obtain the... |
We study a Brownian motor, based on cold atoms in optical lattices, where atomic motion can be induced in a controlled manner in an arbitrary direction, by rectification of isotropic random fluctuations. In contrast with ratchet mechanisms, our Brownian motor operates in a potential that is spatially and temporally sy... |
The effect of spontaneous breaking of initial SO(3) symmetry is shown to be possible for an H-like atom in the ground state, when it is confined in a spherical box under general boundary conditions of "not going out" through the box surface (i.e. third kind or Robin's ones), for a wide range of physically r... |
Recent advances in quantum information processing with trapped ions have demonstrated the need for new ion trap architectures capable of holding and manipulating chains of many (>10) ions. Here we present the design and detailed characterization of a new linear trap, microfabricated with scalable complementary meta... |
The perturbed relativistic coupled-cluster (PRCC) theory is applied to calculate the electric dipole polarizabilities of alkaline Earth metal atoms. The Dirac-Coulomb-Breit atomic Hamiltonian is used and we include the triple excitations in the relativistic coupled-cluster (RCC) theory. |
We demonstrate quantum entanglement of two trapped atomic ion qubits using a sequence of ultrafast laser pulses. Unlike previous demonstrations of entanglement mediated by the Coulomb interaction, this scheme does not require confinement to the Lamb-Dicke regime and can be less sensitive to ambient noise due to its sp... |
Resonant enhancement of high harmonic generation can be obtained in plasmas containing ions with strong radiative transitions resonant with harmonic orders. The mechanism for this enhancement is still debated. |
We study light coherent transport in the weak localization regime using magneto-optically cooled strontium atoms. The coherent backscattering cone is measured in the four polarization channels using light resonant with a J=0 to J=1 transition of the Strontium atom. |
We describe a diabatic protocol to prepare a strongly-interacting Bose-Einstein condensate in a regime where neither an adiabatic ramp nor a direct diabatic quench are desirable. This protocol is expected to achieve a nearly unit population transfer to the strongly-interacting ground state for realistic experimental p... |
Here we report on measurements of the absolute absorption spectra of dense rubidium vapour on the D1 line in the weak-probe regime for temperatures up to 170 C and number densities up to 3 \times 10^14 cm^-3. In such vapours, modifications to the homogeneous linewidth of optical transitions arise due to dipole-dipole ... |
Auger LMM spectra and preliminary model simulations of Ar(9+) and metastable Ar(8+) ions interacting with a clean monocrystalline n-doped Si(100) surface are presented. By varying the experimental parameters, several yet undiscovered spectroscopic features have been observed providing valuable hints for the developmen... |
Nuclear quadrupole moments ($Q$s) in three isotopes of potassium (K) with atomic mass numbers 39, 40 and 41 are evaluated more precisely in this work. The $Q$ value of $^{39}$K is determined to be 0.0614(6) $b$ by combining the available experimental result of the electric quadrupole hyperfine structure constant ($B$)... |
Accurate knowledge of interaction potentials among the alkali atoms and alkaline earth ions is very useful in the studies of cold atom physics. Here we carry out theoretical studies of the long-range interactions among the Li, Na, K, and Rb alkali atoms with the Ca$^+$, Ba$^+$, Sr$^+$, and Ra$^+$ alkaline earth ions s... |
We present an all-optical method to measure and compensate for residual magnetic fields present in a cloud of ultracold atoms trapped in an optical dipole trap. Our approach leverages the increased loss from the trapped atomic sample through electromagnetically induced absorption. |
We investigate the behaviour of electric fields originating from adsorbates deposited on a cryogenic atom chip as it is cooled from room temperature to cryogenic temperature. Using Rydberg electromagnetically induced transparency we measure the field strength versus distance from a 1 mm square of YBCO patterned onto a... |
We investigate the quantum behavior of a mesoscopic two-boson system produced by number-squeezing ultracold gases of alkali metal atoms. The quantum Poincare maps of the wavefunctions are affected by chaos in those regions of the phase space where the classical dynamics produces features that are comparable to hbar. |
We discuss the role of the so-called Darwin-Foldy term in the evaluation of the proton and deuteron charge radii from atomic hydrogen spectroscopy and nuclear scattering data. The question of whether this term should be included or excluded from the nuclear radius has been controversially discussed in the literature. |
Using a laser that is frequency-locked to a Fabry-Perot etalon of high finesse and stability, we probe the 5d10 6s 2S_1/2 (F=0) - 5d9 6s 2D_5/2 (F=2) Delta-m_F = 0 electric-quadrupole transition of a single laser-cooled 199Hg+ ion stored in a cryogenic radio-frequency ion trap. We observe Fourier-transform limited lin... |
We present precise values of the dipole polarizabilities ($\alpha$) of the ground $\rm [4f^{14}6s] ~ ^2S_{1/2}$ and metastable $\rm [4f^{14} 5d] ~ ^2D_{3/2}$ states of Yb$^+$, that are %vital {\bf important} in reducing systematics in the clock frequency of the $\rm[4f^{14}6s] ~ ^2S_{1/2} \rightarrow [4f^{14}5d] ~ ^2D_... |
In this paper we study theoretically the process of electron capture between one-optical-electron atoms (e.g. hydrogenlike or alkali atoms) and ions at low-to-medium impact velocities ($v/v_e \approx 1$) working on a modification of an already developed classical In this work we present an improvement over the Over Bar... |
The progress in optical clock with uncertainty at a level of $10^{-18}$ requires unprecedented precision in estimating the contribution of multipolar and higher-order effects of atom-field interactions. Current theoretical and experimental results of dynamic multipolar polarizabilities and hyperpolarizabilities at the... |
We propose and explore the feasibility of a novel Ramsey interferometer created by a trapped two-state Bose-Einstein condensate (BEC) driven by dipole oscillations and gravitational sag. The BEC is formed in a pure cigar shaped compressed magnetic trap (CMT) via a dilute atom cloud of $^{87}Rb$ atoms in state $\vert F... |
The $^1\mathrm{S}_0$-$^3\mathrm{P}_0$ clock transition frequency $\nu_\text{Sr}$ in neutral $^{87}$Sr has been measured relative to the Cs standard by three independent laboratories in Boulder, Paris, and Tokyo over the last three years. The agreement on the $1\times 10^{-15}$ level makes $\nu_\text{Sr}$ the best agre... |
Photoionization spectra of Se have been studied by step-wise resonance laser ionization. The Rydberg series 4s$^2$4p$^3$($^4$S)np $^3$P$_{0,1,2}$ and 4s$^2$4p$^3$($^4$S)np $^5$P$_{1,2,3}$ were measured via different excitation schemes. |
We report coherent association of atoms into a single weakly bound NaCs molecule in an optical tweezer through an optical Raman transition. The Raman technique uses a deeply bound electronic excited intermediate state to achieve a large transition dipole moment while reducing photon scattering. |
Double photoelectron emission from He atoms by intense laser pulses with a wave length of $394.5\,nm$ is computed for intensities $3.5 - 9.2\times 10^{14}W/cm^2$. Joint momentum distributions confirm the characteristics seen in classical trajectory calculations. |
We show that resonant dipole-dipole interactions between Rydberg atoms in a triangular lattice can give rise to artificial magnetic fields for spin excitations. We consider the coherent dipole-dipole coupling between $np$ and $ns$ Rydberg states and derive an effective spin-1/2 Hamiltonian for the $np$ excitations. |
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