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= = Original design = =
The Type 1 gold dollar depicts a head of Liberty , facing left , with a coronet or tiara on her head bearing her name . Her hair is gathered in a bun ; she is surrounded by 13 stars representing the original states . The reverse features the date and denomination within a wreath , with the name of the nation near the ...
Contemporary reviews of the Type 1 design were generally favorable . The New York Weekly Tribune on May 19 , 1849 described the new dollar as " undoubtedly the neatest , tiniest , lightest , coin in this country ... it is too delicate and beautiful to pay out for potatoes , and sauerkraut , and salt pork . Oberon migh...
= = Modifications = =
Mint records indicate the first gold dollars were produced on May 7 , 1849 ; Longacre 's diary notes state instead that the first were struck on May 8 . A few coins in proof condition were struck on the first day , along with about 1 @,@ 000 for circulation . There are five major varieties of the 1849 gold dollar from...
The continued flow of gold from California made silver expensive in terms of gold , and U.S. silver coins began to flow out of the country for melting in 1849 , a flow that accelerated over the next several years as the price of the metal continued to rise . By 1853 , a thousand dollars in silver coin contained $ 1 @,...
As early as 1851 , New York Congressman William Duer alleged that that Patterson had made the gold dollar too small in diameter on purpose to provoke criticism . Patterson retired that year after 16 years in his position , and under his successor , George N. Eckert , annular gold dollar and half dollar patterns were s...
The Act of February 21 , 1853 , that had lightened the silver coins also authorized a gold three @-@ dollar piece , which began to be produced in 1854 . To ensure that the three @-@ dollar piece was not mistaken for other gold coins , it had been made thinner and wider than it would normally be , and Longacre put a di...
Nevertheless , the Type 2 gold dollar ( as it came to be known ) proved unsatisfactory as the mints had difficulty in striking the new coin so that all details were brought out . This was due to the high relief of the design β€” the three Southern branch mints especially had trouble with the piece . Many of the Type 2 p...
= = = Design of Type 2 and 3 dollars = = =
The Type 2 and 3 gold dollars depict Liberty as a Native American princess , with a fanciful feathered headdress not resembling any worn by any Indian tribe . This image is an inexact copy of the design Longacre had made for the three @-@ dollar piece , and is one of a number of versions of Liberty Longacre created ba...
Art historian Cornelius Vermeule deprecated the Indian princess design used by Longacre for the obverses of the Types 2 and 3 gold dollar , and for the three @-@ dollar piece , " the ' princess ' of the gold coins is a banknote engraver 's elegant version of folk art of the 1850s . The plumes or feathers are more like...
= = War years = =
The gold dollar continued to be produced in the late 1850s , though mintages declined from the figures of two million or more each year between 1850 and 1854 . Only about 51 @,@ 000 gold dollars were produced in 1860 , with over two @-@ thirds of that figure at Philadelphia , just under a third at San Francisco , and ...
The other candidate for the rarest from that mint is the 1861 @-@ D , with an estimated mintage of 1 @,@ 000 and perhaps 45 to 60 known . Two pairs of dies were shipped from Philadelphia to Dahlonega on December 10 , 1860 ; they arrived on January 7 , 1861 , two weeks before Georgia voted to secede from the Union , as...
Dahlonega , like the other two branch mints in the South , closed its doors after the 1861 strikings . It and the Charlotte facility never reopened ; the New Orleans Mint again struck coins from 1879 to 1909 , but did not strike gold dollars again . After 1861 , the only issuance of gold dollars outside Philadelphia w...
The outbreak of the Civil War shook public confidence in the Union , and citizens began hoarding specie , gold and silver coins . In late December 1861 , banks and then the federal Treasury stopped paying out gold at face value . By mid @-@ 1862 , all federal coins , even the base metal cent , had vanished from commer...
= = Final years , abolition , and collecting = =
Since gold did not circulate in the United States ( except on the West Coast ) in the postwar period , much of the production of coins of that metal in the United States was double eagles for export . Accordingly , although 1 @,@ 361 @,@ 355 gold dollars were struck in 1862 β€” the last time production would exceed a mi...
In the 1870s and 1880s , public interest grew in the low @-@ mintage gold dollar . Collecting coins was becoming more popular , and a number of numismatists put aside some gold dollars and hoped for increases in value . The Mint most likely channeled its production through some favored Philadelphia dealers , though pr...
James Pollock , in his final report as Mint Director in 1873 , advocated limiting striking of gold dollars to depositors who specifically requested it . " The gold dollar is not a convenient coin , on account of its small size , and it suffers more proportionately from abrasion than larger coins . " His successors cal...
A total of 19 @,@ 499 @,@ 337 gold dollars were coined , of which 18 @,@ 223 @,@ 438 were struck at Philadelphia , 1 @,@ 004 @,@ 000 at New Orleans , 109 @,@ 138 at Charlotte , 90 @,@ 232 at San Francisco and 72 @,@ 529 at Dahlonega . According to an advertisement in the February 1899 issue of The Numismatist , gold d...
= = Commemorative gold dollars = =
The gold dollar had a brief resurrection during the period of Early United States commemorative coins . Between 1903 and 1922 nine different issues were produced , with a total mintage of 99 @,@ 799 . These were minted for various public events , did not circulate , and none used Longacre 's design .
= Johnson – Corey – Chaykovsky reaction =
The Johnson – Corey – Chaykovsky reaction ( sometimes referred to as the Corey – Chaykovsky reaction or CCR ) is a chemical reaction used in organic chemistry for the synthesis of epoxides , aziridines , and cyclopropanes . It was discovered in 1961 by A. William Johnson and developed significantly by E. J. Corey and ...
The reaction is most often employed for epoxidation via methylene transfer , and to this end has been used in several notable total syntheses ( See Synthesis of epoxides below ) . Additionally detailed below are the history , mechanism , scope , and enantioselective variants of the reaction . Several reviews have been...
= = History = =
The original publication by Johnson concerned the reaction of 9 @-@ dimethylsulfonium fluorenylide with substituted benzaldehyde derivatives . The attempted Wittig @-@ like reaction failed and a benzalfluorene oxide was obtained instead , noting that " Reaction between the sulfur ylid and benzaldehydes did not afford ...
The subsequent development of ( dimethyloxosulfaniumyl ) methanide , ( CH3 ) 2SOCH2 and ( dimethylsulfaniumyl ) methanide , ( CH3 ) 2SCH2 ( known as Corey – Chaykovsky reagents ) by Corey and Chaykovsky as efficient methylene @-@ transfer reagents established the reaction as a part of the organic canon .
= = Mechanism = =
The reaction mechanism for the Johnson – Corey – Chaykovsky reaction consists of nucleophilic addition of the ylide to the carbonyl or imine group . A negative charge is transferred to the heteroatom and because the sulfonium cation is a good leaving group it gets expelled forming the ring . In the related Wittig reac...
The trans diastereoselectivity observed results from the reversibility of the initial addition , allowing equilibration to the favored anti betaine over the syn betaine . Initial addition of the ylide results in a betaine with adjacent charges ; density functional theory calculations have shown that the rate @-@ limit...
The degree of reversibility in the initial step ( and therefore the diastereoselectivity ) depends on four factors , with greater reversibility corresponding to higher selectivity :
Stability of the substrate with higher stability leading to greater reversibility by favoring the starting material over the betaine .
Stability of the ylide with higher stability similarly leading to greater reversibility .
Steric hindrance in the betaine with greater hindrance leading to greater reversibility by disfavoring formation of the intermediate and slowing the rate @-@ limiting rotation of the central bond .
Solvation of charges in the betaine by counterions such as lithium with greater solvation allowing more facile rotation in the betaine intermediate , lowering the amount of reversibility .
= = Scope = =
The application of the Johnson – Corey – Chaykovsky reaction in organic synthesis is diverse . The reaction has come to encompass reactions of many types of sulfur ylides with electrophiles well beyond the original publications . It has seen use in a number of high @-@ profile total syntheses , as detailed below , and...
= = = Types of ylides = = =
Many types of ylides can be prepared with various functional groups both on the anionic carbon center and on the sulfur . The substitution pattern can influence the ease of preparation for the reagents ( typically from the sulfonium halide , e.g. trimethylsulfonium iodide ) and overall reaction rate in various ways . ...
Use of a sulfoxonium allows more facile preparation of the reagent using weaker bases as compared to sulfonium ylides . ( The difference being that a sulfoxonium contains a doubly bonded oxygen whereas the sulfonium does not . ) The former react slower due to their increased stability . In addition , the dialkylsulfox...
The vast majority of reagents are monosubstituted at the ylide carbon ( either R1 or R2 as hydrogen ) . Disubstituted reagents are much rarer but have been described :
If the ylide carbon is substituted with an electron @-@ withdrawing group ( EWG ) , the reagent is referred to as a stabilized ylide . These , similarly to sulfoxonium reagents , react much slower and are typically easier to prepare . These are limited in their usefulness as the reaction can become prohibitively slugg...
If the ylide carbon is substituted with an aryl or allyl group , the reagent is referred to as a semi @-@ stabilized ylide . These have been developed extensively , second only to the classical methylene reagents ( R1 = R2 = H ) . The substitution pattern on aryl reagents can heavily influence the selectivity of the r...
If the ylide carbon is substituted with an alkyl group the reagent is referred to as an unstabilized ylide . The size of the alkyl groups are the major factors in selectivity with these reagents .
The R @-@ groups on the sulfur , though typically methyls , have been used to synthesize reagents that can perform enantioselective variants of the reaction ( See Variations below ) . The size of the groups can also influence diastereoselectivity in alicyclic substrates .
= = = Synthesis of epoxides = = =
Reactions of sulfur ylides with ketones and aldehydes to form epoxides are by far the most common application of the Johnson – Corey – Chaykovsky reaction . Examples involving complex substrates and ' exotic ' ylides have been reported , as shown below .
The reaction has been used in a number of notable total syntheses including the Danishefsky Taxol total synthesis , which produces the chemotherapeutic drug taxol , and the Kuehne Strychnine total synthesis which produces the pesticide strychnine .
= = = Synthesis of aziridines = = =
The synthesis of aziridines from imines is another important application of the Johnson – Corey – Chaykovsky reaction and provides an alternative to amine transfer from oxaziridines . Though less widely applied , the reaction has a similar substrate scope and functional group tolerance to the carbonyl equivalent . The...
= = = Synthesis of cyclopropanes = = =
For addition of sulfur ylides to enones , higher 1 @,@ 4 @-@ selectivity is typically obtained with sulfoxonium reagents than with sulfonium reagents . Many electron @-@ withdrawing groups have been shown compatible with the reaction including ketones , esters , and amides ( the example below involves a Weinreb amide ...
= = = Other reactions = = =
In addition to the reactions originally reported by Johnson , Corey , and Chaykovsky , sulfur ylides have been used for a number of related homologation reactions that tend to be grouped under the same name .
With epoxides and aziridines the reaction serves as a ring @-@ expansion to produce the corresponding oxetane or azetidine . The long reaction times required for these reactions prevent them from occurring as significant side reactions when synthesizing epoxides and aziridines .
Several cycloadditions wherein the ylide serves as a " nucleophilic carbenoid equivalent " have been reported .
Living polymerizations using trialkylboranes as the catalyst and ( dimethyloxosulfaniumyl ) methanide as the monomer have been reported for the synthesis of various complex polymers .
= = Enantioselective variations = =
The development of an enantioselective ( i.e. yielding an enantiomeric excess , which is labelled as " ee " ) variant of the Johnson – Corey – Chaykovsky reaction remains an active area of academic research . The use of chiral sulfides in a stoichiometric fashion has proved more successful than the corresponding catal...
= = = Stoichiometric reagents = = =
The most successful reagents employed in a stoichiometric fashion are shown below . The first is a bicyclic oxathiane that has been employed in the synthesis of the Ξ² @-@ adrenergic compound dichloroisoproterenol ( DCI ) but is limited by the availability of only one enantiomer of the reagent . The synthesis of the ax...
The other major reagent is a camphor @-@ derived reagent developed by Varinder Aggarwal of the University of Bristol . Both enantiomers are easily synthesized , although the yields are lower than for the oxathiane reagent . The ylide conformation is determined by interaction with the bridgehead hydrogens and approach ...