Daily Papers

The recent discovery of relaxor ferroelectricity and magnetoelectric effect in lightly doped cuprate material La_2CuO_{4+x} has provided a number of questions concerning its theoretical description. It has been argued using a Ginzburg-Landau free energy approach that the magnetoelectric effect can be explained by the presence of bi-quadratic interaction terms in the free energy. Here, by using the same free energy functional, we study the variety of behavior which can emerge in the electric polarization under an external magnetic field. Subsequently, we discuss the role of Dzyaloshinskii-Moriya interaction in generating this magnetoelectric response. This work is particularly relevant for such relaxor systems where the material-dependent parameters would be affected by changes in e.g. chemical doping or cooling rate.

The strong coupling between magnetism and ferroelectricity was found in rare earth manganites, where the electric polarization could be induced by special magnetic ordering. There is no theoretical model that would allow us to study the static and dynamic properties of electric polarization in strongly correlated magnetic dielectrics. In the presented research, we have taken the main step towards the construction of such a fundamental model, and made a direct connection between the microscopic Katsura-Nagaosa-Balatsky theory and Mostovoy's phenomenological model for magnetically induced polarization. A novel description of the ferroelectricity of spin origin is proposed within the framework of the many-particle quantum hydrodynamics method. It is applied to the study of cells of magnetic ions, where the electric dipole moment is proportional to the vector product of spins. Our approach is based on the many-particle Pauli equation, where the influence of an external magnetic field is considered. We define the electric dipole moment operator of the ion cell and introduce the macroscopic polarization as the quantum mechanical average of that operator. We formulate a model for the description of nonequilibrium polarization and derive a new polarization evolution equation. The polarization switching in ferroelectric magnets with the spiral spin-density-wave state is considered, and we demonstrate that the proposed model yields known results and can predict novel effects. The dynamic magnetoelectric effect can be investigated by employing this novel equation to study the evolution of polarization.

In a recent study Viskadourakis et al. discovered that extremely underdoped La_2CuO_(4+x) is a relaxor ferroelectric and a magnetoelectric material at low temperatures. It is further observed that the magnetoelectric response is anisotropic for different directions of electric polarization and applied magnetic field. By constructing an appropriate Landau theory, we show that a bi-quadratic magnetoelectric coupling can explain the experimentally observed polarization dependence on magnetic field. This coupling leads to several novel low-temperature effects including a feedback enhancement of the magnetization below the ferroelectric transition, and a predicted magnetocapacitive effect.

Autferroics, recently proposed as a sister branch of multiferroics, exhibit strong intrinsic magnetoelectricity, but ferroelectricity and magnetism are mutually exclusive rather than coexisting. Here, a general model is considered based on the Landau theory, to clarify the distinction between multi and autferroics by qualitative change-rotation in Landau free energy landscape and in particular phase mapping. The TiGeSe_3 exemplifies a factual material, whose first-principles computed Landau coefficients predict its autferroicity. Our investigations pave the way for an alternative avenue in the pursuit of intrinsically strong magnetoelectrics.

Axion insulators possess a quantized axion field theta=pi protected by combined lattice and time-reversal symmetry, holding great potential for device applications in layertronics and quantum computing. Here, we propose a high-spin axion insulator (HSAI) defined in large spin-s representation, which maintains the same inherent symmetry but possesses a notable axion field theta=(s+1/2)^2pi. Such distinct axion field is confirmed independently by the direct calculation of the axion term using hybrid Wannier functions, layer-resolved Chern numbers, as well as the topological magneto-electric effect. We show that the guaranteed gapless quasi-particle excitation is absent at the boundary of the HSAI despite its integer surface Chern number, hinting an unusual quantum anomaly violating the conventional bulk-boundary correspondence. Furthermore, we ascertain that the axion field theta can be precisely tuned through an external magnetic field, enabling the manipulation of bonded transport properties. The HSAI proposed here can be experimentally verified in ultra-cold atoms by the quantized non-reciprocal conductance or topological magnetoelectric response. Our work enriches the understanding of axion insulators in condensed matter physics, paving the way for future device applications.

With copper-substituted lead apatite below room temperature, we observe diamagnetic dc magnetization under magnetic field of 25 Oe with remarkable bifurcation between zero-field-cooling and field-cooling measurements, and under 200 Oe it changes to be paramagnetism. A glassy memory effect is found during cooling. Typical hysteresis loops for superconductors are detected below 250 K, along with an asymmetry between forward and backward sweep of magnetic field. Our experiment suggests at room temperature the Meissner effect is possibly present in this material.

A new multiferroic material, CuBr2, is reported for the first time. CuBr2 has not only a high transition temperature (close to liquid nitrogen temperature) but also low dielectric loss and strong magnetoelectric coupling. These findings reveal the importance of anion effects in the search for the high temperature multiferroics materials among these low-dimensional spin systems.

Recently we have reported the observation of colossal magnetostriction effect in HoMn2O5 single crystals. Besides we have made the supposition for possible correlation between the peculiarities, observed in the field depended polarization measurements, and the colossal magnetostriction effect at a 4.2 K temperature. In this article we present our results received by polarization and magnetostriction measurements on HoMn2O5 and TbMn2O5 single crystals and the strong correlation between magnetostriction and polarization phase transition for these two compounds. The origin of this correlation is discussed.

A large transverse thermoelectric response, known as anomalous Nernst effect (ANE) has been recently observed in several topological magnets. Building a thermopile employing this effect has been the subject of several recent propositions. Here, we design and build a thermopile with an array of tilted adjacent crystals of Mn_3Sn. The design employs a single material and replaces pairs of P and N thermocouples of the traditional design with hermaphroditic legs. The design exploits the large lag angle between the applied field and the magnetization, which we attribute to the interruption of magnetic octupoles at the edge of xy-plane. Eliminating extrinsic contacts between legs will boost the efficiency, simplify the process and pave the way for a new generation of thermopiles.

We report the discovery of a ferroelectric ground state below 4.5 K in highly underdoped La_2CuO_(4+x) accompanied by slow charge dynamics which develop below T~40 K. An anisotropic magnetoelectric response has also been observed, indicating considerable spin-charge coupling in this lightly doped "parent" high temperature copper-oxide superconductor. The ferroelectric state is proposed to develop from polar nanoregions, in which spatial inversion symmetry is locally broken due to non-stoichiometric carrier doping.

We show that PT-symmetry acts as the effective time-reversal symmetry governing Anderson localization in the antiferromagnet BaMn_2Bi_2, whereas the general time-reversal symmetry is broken by its long-range magnetic order. The magnetoconductance follows the laws established from breaking time-reversal symmetry throuhg the orbital coupling of charge carriers to the magnet vector potential, however, the degrees of symmetry breaking are qualitatively modulated by the magnetocrystalline anisotropy stabilizing PT-related sublattices. The quantum interferences and hoping amplitudes governing the phenomena are drastically impaired by transverse magnetic fields, which readily cant PT-related magnetic sublattices. Accordingly, when the PT-related texture is weakly perturbed by longitudinal fields orienting along the sublattices, the localization is minutely affected. The robustness of the PT-enforced degeneracies is thus governed by exchange and magnetocrystalline interactions, in contrast to the exact PT-symmetry of the full Hamiltonian, which is broken by any finite field.

We numerically investigate some properties of unbalanced St\"{u}ckelberg holographic superconductors, by considering backreaction effects of fields on the background geometry. More precisely, we study the impacts of the chemical potential mismatch and St\"{u}ckelberg mechanism on the condensation and conductivity types (electrical, spin, mixed, thermo-electric, thermo-spin and thermal conductivity). Our results show that the St\"{u}ckelberg's model parameters C_{alpha} and alpha not only have significant impacts on the phase transition, but also affect the conductivity pseudo-gap and the strength of conductivity fluctuations. Moreover, the effects of these parameters on a system will be gradually reduced as the imbalance grows. We also find that the influence of alpha on the amplitude of conductivity fluctuations depends on the magnitude of the both C_{alpha} and deltamu/mu in the electric and thermal conductivity cases. This results in that increasing alpha can damp the conductivity fluctuations of an unbalanced system in contrast to balanced ones.

We successfully synthesized a novel intermetallic compound rm CrFe_2Ge_2 with the rm Fe_{13}Ge_{8}-type crystal structure. A structural study is presented combining single-crystal X-ray diffraction and Mössbauer spectroscopy analysis, confirming the presence of two distinct Fe sublattices. rm CrFe_2Ge_2 exhibits a metallic ferromagnetic state with T_C approx rm 200~K. This material does not follow the usual M^2 propto H/M Arrott law, rather a modified Arrott law is obeyed in this material. The critical exponents determined from detailed analysis of modified Arrott plots were found to be β= 0.392, γ= 1.309 and δ= 4.26 obtained from the critical isotherm at T_{rm C} =rm 200~K. Self-consistency and reliability of the critical exponent analysis were verified by the Widom scaling law and scaling equations. Using the results from renormalization group calculation, the critical behavior of rm CrFe_2Ge_2 is akin to that of a d=3, n=3 ferromagnet in which the magnetic exhange distance is found to decay as J(r) approx r^{-4.86} with long-range magnetic coupling. The evaluated Rhodes-Wohlfarth ratio of sim 3 points to an itinerant ferromagnetic ground state. Low-temperature measurements of resistivity, p(T), and specific heat, C_P(T), reveal a pronounced contribution from electron-magnon scattering.

We present a comprehensive numerical study of a six-state clock model with a long-range dipolar type interaction. This model is motivated by the ferroelectric orders in the multiferroic hexagonal manganites. At low temperatures, trimerization of local atomic structures leads to six distinct but energetically degenerate structural distortion, which can be modeled by a six-state clock model. Moreover, the atomic displacements in the trimerized state further produce a local electric polarization whose sign depends on whether the clock variable is even or odd. These induced electric dipoles, which can be modeled by emergent Ising degrees of freedom, interact with each other via long-range dipolar interactions. Extensive Monte Carlo simulations are carried out to investigate low temperature phases resulting from the competing interactions. Upon lowering temperature, the system undergoes two Berezinskii-Kosterlitz-Thouless (BKT) transitions, characteristic of the standard six-state clock model in two dimensions. The dipolar interaction between emergent Ising spins induces a first-order transition into a ground state characterized by a three-fold degenerate stripe order. The intermediate phase between the discontinuous and the second BKT transition corresponds to a maze-like hexagonal liquid with short-range stripe ordering. Moreover, this intermediate phase also exhibits an unusual ferromagnetic order with two adjacent clock variables occupying the two types of stripes of the labyrinthine pattern.

A cylindrical TM_{0,1,0} mode microwave cavity resonator was excited using a balanced interferometric configuration that allowed manipulation of the electric field and potential within the resonator by adjusting the phase and amplitude of the interferometer arms driving the resonator. With precise tuning of the phase and amplitude, 25 dB suppression of the electric field at the resonance frequency was achieved while simultaneously resonantly enhancing the time-varying electric-scalar potential. Under these conditions, the system demonstrated electromagnetically induced absorption in the cavity response due to the annulment of the electric field at the resonance frequency. This phenomena can be regarded as a form of extreme dispersion, and led to a sharp increase in the cavity phase versus frequency response by an order of magnitude when compared to the cavity Q-factor. This work presents an experimental setup that will allow the electric-scalar Aharonov-Bohm effect to be tested under conditions involving a time-varying electric-scalar potential, without the presence of an electric field or magnetic vector potential, an experiment that has not yet been realised.

A domain wall (DW) which moves parallel to a magnetically compensated interface between an antiferromagnetic insulator (AFMI) and a two-dimensional (2D) metal can pump spin polarization into the metal. It is assumed that localized spins of a collinear AFMI interact with itinerant electrons through their exchange interaction on the interface. We employed the formalism of Keldysh Green's functions for electrons which experience potential and spin-orbit scattering on random impurities. This formalism allows a unified analysis of spin pumping, spin diffusion and spin relaxation effects on a 2D electron gas. It is shown that the pumping of a nonstaggered magnetization into the metal film takes place in the second order with respect to the interface exchange interaction. At sufficiently weak spin relaxation this pumping effect can be much stronger than the first-order effect of the Pauli magnetism which is produced by the small nonstaggered exchange field of the DW. It is shown that the pumped polarization is sensitive to the geometry of the electron's Fermi surface and increases when the wave vector of the staggered magnetization approaches the nesting vector of the Fermi surface. In a disordered diffusive electron gas the induced spin polarization follows the motion of the domain wall. It is distributed asymmetrically around the DW over a distance which can be much larger than the DW width.

Alloys with a first-order magnetic transition are central to solid-state refrigeration technology, sensors and actuators, or spintronic devices. The discontinuous nature of the transition in these materials is a consequence of the coupling between the magnetic, electronic and structural subsystems, but in a real experiment, it is difficult to observe and analyze the simultaneous evolution of all the subsystems. As a result, it is very hard to determine the main mechanisms of the transition and purposefully develop these advanced magnetic materials. To resolve this issue, we changed the existing paradigm and conducted simultaneous measurements of the macroscopic properties - magnetization, temperature change of the sample, longitudinal and transversal magnetostrictions - to reveal the rich details of the magneto-structural, first-order transition occurring in the prototypical alloy LaFe11.8Si1.2. We complement these findings with experiments on the atomistic scale, i.e., x-ray absorption spectroscopy (XAS), x-ray magnetic circular dichroism (XMCD) and Mössbauer spectroscopy, and then combine them with first-principles calculations to reveal the full complexity and two-stage nature of the transition. This new approach can be successfully extended to a large class of advanced magnetic materials that exhibit analogous transformations.

Symmetry has long provided the organizing principle for understanding how materials respond to external perturbations. Here we show that what is permitted by symmetry need not be what actually emerges from the underlying system, and this distinction becomes particularly consequential for symmetry-related gapless Dirac fermions such as in altermagnets. A perturbation that shifts the Dirac points drives a Lifshitz reconstruction and generates an intrinsically nonanalytic effective potential, giving rise to undiscovered singular responses. In Dirac altermagnets, this nonanalyticity acquires a magnetic manifestation through C-paired spin-polarized Dirac cones: breaking the pairing symmetry C lifts their degeneracy and converts the associated Lifshitz reconstruction into an itinerant magnetization. As a consequence, piezomagnetism, the induction of a net magnetization by a mechanical strain, becomes nonlinear and nonanalytic, with Mproptosgn(varepsilon)varepsilon^2, whereas the linear response is absent despite being allowed by symmetry. Accordingly, the leading response cannot be inferred from the conventional symmetry-based paradigm of material response built upon the cornerstones of Neumann's principle and analytic Landau expansion. First-principles calculations identify the monolayer Fe_2S as a candidate material realization for such singular magnetic responses. These results suggest quantum singularities as a new degree of freedom for engineering material responses.

We describe the first-principles design and subsequent synthesis of a new material with the specific functionalities required for a solid-state-based search for the permanent electric dipole moment of the electron. We show computationally that perovskite-structure europium barium titanate should exhibit the required large and pressure-dependent ferroelectric polarization, local magnetic moments, and absence of magnetic ordering even at liquid helium temperature. Subsequent synthesis and characterization of Eu_{0.5}Ba_{0.5}TiO_3 ceramics confirm the predicted desirable properties.

Hysteresis is more than just an interesting oddity, which occurs in materials with a first-order transition. It is a real obstacle on the path from existing lab-scale prototypes of magnetic refrigerators towards commercialization of this potentially disruptive cooling technology. Indeed, the reversibility of the magnetocaloric effect, being essential for magnetic heat pumps, strongly depends on the width of the thermal hysteresis and therefore it is necessary to understand the mechanisms causing hysteresis and to find solutions how to minimize losses associated with thermal hysteresis in order to maximize the efficiency of magnetic cooling devices. In this work, we discuss fundamental aspects, which can contribute to thermal hysteresis and we are developing strategies for at least partially overcoming the hysteresis problem in some selected classes of magnetocaloric materials with large application potential. Doing so, we refer to the most relevant classes of magnetic refrigerants La-Fe-Si-, Heusler- and Fe2P-type compounds.

The discovery of van der Waals magnets has established a new domain in the field of magnetism, opening novel pathways for the electrical control of magnetic properties. In this context, Fe3GeTe2 (FGT) emerges as an exemplary candidate owing to its intrinsic metallic properties, which facilitate the interplay of both charge and spin degrees of freedom. Here, the bidirectional voltage control of exchange bias (EB) effect in a perpendicularly magnetized all-van der Waals FGT/O-FGT/hBN heterostructure is demonstrated. The antiferromagnetic O-FGT layer is formed by naturally oxidizing the FGT surface. The observed EB magnitude reaches 1.4 kOe with a blocking temperature (150 K) reaching close to the Curie temperature of FGT. Both the exchange field and the blocking temperature values are among the highest in the context of layered materials. The EB modulation exhibits a linear dependence on the gate voltage and its polarity, observable in both positive and negative field cooling (FC) experiments. Additionally, gate voltage-controlled magnetization switching, highlighting the potential of FGT-based heterostructures is demonstrated in advanced spintronic devices. These findings display a methodology to modulate the magnetism of van der Waals magnets offering new avenues for the development of high-performance magnetic devices.

The optical properties of the superconducting K_{0.8}Fe_{1.7}(Se_{0.73}S_{0.27})_2 single crystals with a critical temperature T_capprox 26 K have been measured in the {\it ab} plane in a wide frequency range using both infrared Fourier-transform spectroscopy and spectroscopic ellipsometry at temperatures of 4--300 K. The normal-state reflectance of K_{0.8}Fe_{1.7}(Se_{0.73}S_{0.27})_2 is analyzed using a Drude-Lorentz model with one Drude component. The temperature dependences of the plasma frequency, optical conductivity, scattering rate, and dc resistivity of the Drude contribution in the normal state are presented. In the superconducting state, we observe a signature of the superconducting gap opening at 2Δ(5~K) = 11.8~meV. An abrupt decrease in the low-frequency dielectric permittivity varepsilon _1(ω) at T < T_c also evidences the formation of the superconducting condensate. The superconducting plasma frequency ω_{pl,s} = (213pm 5)~cm^{-1} and the magnetic penetration depth λ=(7.5pm 0.2)~μm at T=5~K are determined.

The emergence of spin-polarized electrons from nonmagnetic chiral molecules and crystals is called Chirality-induced spin selectivity (CISS). A chiral phonon of definite wavevector q can strongly enhance it, but near equilibrium the two helicities +q and -q are equally populated: they are time-reversal partners and their contributions cancel. We show that in a biased chiral conductor the current causes the phonon of one helicity to damp less than the other. The damping asymmetry is odd in the current, odd under qrightarrow-q, invariant under a mirror that reverses the structural handedness, and equal, mode for mode, to the current-induced nonconservative Berry force on the phonon coordinate. Closing the phonon kinetics with a rate equation turns the asymmetry into a net lattice helicity: at any finite bias one helicity is preferentially populated, with no threshold, growing linearly with the current as Vrightarrow0; above a threshold that helicity becomes a self-sustained coherent travelling wave. We demonstrate this effect in elemental tellurium, treated as an open quantum system (electronic Hamiltonian, phonon bath, and electron-phonon coupling) within a quasi-ab initio framework. The electronic Hamiltonian is supplied by a vertex-corrected quasiparticle self-consistent GW (QSGW) potential with spin-orbit coupling; nuclear displacements are modeled with a machine-learned interatomic potential, which yields chiral phonon modes at finite pm q_z on the Γ-A line. The perturbation to the electronic Hamiltonian from a nuclear displacement is approximated by a frozen-phonon deformation potential. No optical pump is needed: a bias alone drives the current and selects the phonon helicity; reversing the current reverses the selection.

The magnetization in a superconductor induced due to the inverse proximity effect is investigated in hybrid bilayers containing a superconductor and a ferromagnetic insulator or a strongly spin-polarized ferromagnetic metal. The study is performed within a quasiclassical Green function framework, wherein Usadel equations are solved with boundary conditions appropriate for strongly spin-polarized ferromagnetic materials. A comparison with recent experimental data is presented. The singlet to triplet conversion of the superconducting correlations as a result of the proximity effect with a ferromagnet is studied.

We establish, in general terms, the conditions to be satisfied by a time-fractional approach formulation of the Poisson-Nernst-Planck model in order to guarantee that the total current across the sample be solenoidal, as required by the Maxwell equation. Only in this case the electric impedance of a cell can be determined as the ratio between the applied difference of potential and the current across the cell. We show that in the case of anomalous diffusion, the model predicts for the electric impedance of the cell a constant phase element behaviour in the low frequency region. In the parametric curve of the reactance versus the resistance, the slope coincides with the order of the fractional time derivative.

Edge magnetoplasmons (EMPs) provide a platform for probing chiral charge dynamics and nonreciprocal microwave transport in topological quantum materials. However, detecting small perturbations to EMP propagation remains challenging because their signatures in conventional microwave scattering measurements can be weak. Here, we investigate microwave-photon-induced perturbations of EMP transport using a quantum anomalous Hall topological circulator. Pump--probe measurements reveal a strongly frequency-selective response: while microwave irradiation substantially modifies the EMP transmission at several pump frequencies, the transmission remains nearly unchanged at selected frequencies, including 4 and 7 GHz. We further exploit the non-Hermitian mode hybridization of the coupled EMP-resonator system to probe the response near an exceptional point (EP). The pump-induced change in transmission magnitude near the EP is approximately twice that observed away from the EP, demonstrating an enhanced microwave response to perturbations. These results reveal the interplay among chiral EMP transport, microwave-photon-induced perturbations, and non-Hermitian dynamics, and demonstrate the potential of topological circulators as a promising platform for enhanced microwave spectroscopy and sensing.

Hybrid superconductor-semiconductor systems have received a great deal of attention in the last few years because of their potential for quantum engineering, including novel qubits and topological devices. The proximity effect, the process by which the semiconductor inherits superconducting correlations, is an essential physical mechanism of such hybrids. Recent experiments have demonstrated the proximity effect in hole-based semiconductors, but, in contrast to electrons, the precise mechanism by which the hole bands acquire superconducting correlations remains an open question. In addition, hole spins exhibit a complex strong spin-orbit interaction, with largely anisotropic responses to electric and magnetic fields, further motivating the importance of understanding the interplay between such effects and the proximity effect. In this work, we analyze this physics with focus on germanium-based two-dimensional gases. Specifically, we develop an effective theory supported by full numerics, allowing us to extract various analytical expressions and predict different types of superconducting correlations including non-standard forms of singlet and triplet pairing mechanisms with non-trivial momentum dependence; as well as different Zeeman and Rashba spin-orbit contributions. This, together with their precise dependence on electric and magnetic fields, allows us to make specific experimental predictions, including the emergence of f-type superconductivity, Bogoliubov Fermi surfaces, and gapless regimes caused by large in-plane magnetic fields.

In 2021 Nature Physics published a paper by Vaitiekenas, Liu, Krogstrup and Marcus titled "Zero-bias peaks at zero magnetic field in ferromagnetic hybrid nanowires". The paper reports low temperature transport measurements on semiconductor InAs nanowires with two partly overlapping shells -- a shell of EuS, a magnetic insulator, and a shell of Al, a metal that becomes superconducting at temperatures below 1.2K. The paper claims that (1) the data are consistent with induced topological superconductivity and Majorana zero modes (MZMs), and (2) that this is facilitated by the breaking of the time reversal symmetry through a direct magnetic interaction with the EuS shell. In this Matters Arising, we present an alternative explanation which is based on trivial effects that are likely to appear in the reported geometry. Specifically, first, we find that data the authors present in support of the topological superconductivity claim can originate from unintended quantum dots in their devices, a widely known likely explanation that is not being discussed in the paper. Second, our analysis of the setup, supported by our numerical micromagnetic simulations, shows similar effects could be obtained due to stray magnetic fields from the region of the EuS shell damaged during Al etching. This basic picture should come before the exotic interpretation in terms of magnetic exchange interaction with a ferromagnetic insulator.

We have explored, computationally and experimentally, the magnetic properties of alloys. Calculations provide a good agreement with experiment in terms of the saturation magnetization and the magnetocrystalline anisotropy energy with some difficulty in describing Co_2B, for which it is found that both full potential effects and electron correlations treated within dynamical mean field theory are of importance for a correct description. The material exhibits a uniaxial magnetic anisotropy for a range of cobalt concentrations between x=0.1 and x=0.5. A simple model for the temperature dependence of magnetic anisotropy suggests that the complicated non-monotonous temperature behaviour is mainly due to variations in the band structure as the exchange splitting is reduced by temperature. Using density functional theory based calculations we have explored the effect of substitutional doping the transition metal sublattice by the whole range of 5d transition metals and found that doping by Re or W elements should significantly enhance the magnetocrystalline anisotropy energy. Experimentally, W doping did not succeed in enhancing the magnetic anisotropy due to formation of other phases. On the other hand, doping by Ir and Re was successful and resulted in magnetic anisotropies that are in agreement with theoretical predictions. In particular, doping by 2.5~at.\% of Re on the Fe/Co site shows a magnetocrystalline anisotropy energy which is increased by 50\% compared to its parent (Fe_{0.7}Co_{0.3})_2B compound, making this system interesting, for example, in the context of permanent magnet replacement materials or in other areas where a large magnetic anisotropy is of importance.

We carried out numerical simulations of propagation of spin waves (magnons in quantum language) in a yttrium-iron garnet film. The numerical model is based on an original formalism. We demonstrated that a potential barrier for magnons, created by an Oersted field of a dc current flowing through a wire sitting on top of the film, is able to act as an electrically controlled partly transparent mirror for the magnons. We found that the mirror transparency can be set to 50% by properly adjusting the current strength, thus creating a semi-transparent mirror. A strong Hong-Ou-Mandel Effect for single magnons is expected in this configuration. The effect must be seen as two single magnons, launched simultaneously into the film from two transducers located from the opposite sides of the mirror, creating a two-microwave-photon state at the output port of one of the transducers. The probability of seeing those two-photon states at the output port of either transducer must be the same for both transducers.

The inhomogeneous magnetic stray field of micromagnets has been extensively used to manipulate electron spin qubits. By means of micromagnetic simulations and scanning superconducting quantum interference device microscopy, we show that the polycrystallinity of the magnet and non-uniform magnetization significantly impact the stray field and corresponding qubit properties. We find that the random orientation of the crystal axis in polycrystalline Co magnets alters the qubit frequencies by up to 0.5 GHz, compromising single qubit addressability and single gate fidelities. We map the stray field of Fe micromagnets with an applied magnetic field of up to 500 mT (mimicking conditions when operating qubits), finding field gradients above 1 mT/nm. The measured gradients and the lower magnetocrystalline anisotropy of Fe demonstrate the advantage of using Fe instead of Co for magnets in spin qubit devices. These properties of Fe also enabled us to design a 2D arrangement of nanomagnets for driving spin qubits distributed on a 2D lattice.

Electric field control of magnetic properties offers a broad and promising toolbox for enabling ultra-low power electronics. A key challenge with high technological relevance is to master the interplay between the magnetic anisotropy of a ferromagnet and the exchange coupling to an adjacent antiferromagnet. Here, we demonstrate that magneto-ionic gating can be used to achieve a very stable out-of-plane (OOP) oriented magnetization with strong exchange bias in samples with as-deposited preferred in-plane (IP) magnetization. We show that the perpendicular interfacial anisotropy can be increased by more than a factor 2 in the stack Ta/Pt/PtMn/Co/HfO2 by applying -2.5 V gate voltage over 3 nm HfO2, causing a reorientation of the magnetization from IP to OOP with a strong OOP exchange bias of more than 50 mT. Comparing two thicknesses of PtMn, we identify a notable trade-off: while thicker PtMn yields a significantly larger exchange bias, it also results in a slower response to ionic liquid gating within the accessible gate voltage window. These results pave the way for post-deposition electrical tailoring of magnetic anisotropy and exchange bias in samples requiring significant exchange bias.

We report on the impact of magnetoelastic coupling on the magnetocaloric properties of LaFe_{11.4}Si_{1.6}H_{1.6} in terms of the vibrational density of states, which we determined with ^{57}Fe nuclear resonant inelastic X-ray scattering measurements and with density-functional-theory based first-principles calculations in the ferromagnetic low-temperature and paramagnetic high-temperature phase. In experiments and calculations, we observe pronounced differences in the shape of the Fe-partial VDOS between non-hydrogenated and hydrogenated samples. This shows that hydrogen does not only shift the temperature of the first-order phase transition, but also affects the elastic response of the Fe-subsystem significantly. In turn, the anomalous redshift of the Fe VDOS, observed by going to the low-volume PM phase, survives hydrogenation. As a consequence, the change in the Fe specific vibrational entropy ΔS_lat across the phase transition has the same sign as the magnetic and electronic contribution. DFT calculations show that the same mechanism, which is a consequence of the itinerant electron metamagnetism associated with the Fe subsystem, is effective in both the hydrogenated and he hydrogen-free compounds. Although reduced by 50 % as compared to the hydrogen-free system, the measured change ΔS_lat of 3.2\pm1.9 J/kgK across the FM to PM transition contributes with 35 % significantly and cooperatively to the total isothermal entropy change ΔS_iso. Hydrogenation is observed to induce an overall blueshift of the Fe-VDOS with respect to the H-free compound; this effect, together with the enhanced Debye temperature observed, is a fingerprint of the hardening of the Fe sublattice by hydrogen incorporation. In addition, the mean Debye velocity of sound of LaFe_{11.4}Si_{1.6}H_{1.6} was determined from the NRIXS and the DFT data.

In this study, the spin-orbit torque (SOT) in light metal oxide systems is investigated using an experimental approach based on harmonic Hall voltage techniques in out-of-plane (OOP) angular geometry for samples with in-plane magnetic anisotropy. In parallel, an analytical derivation of this alternative OOP harmonic Hall detection geometry has been developed, followed by experimental validation to extract SOT effective fields. In addition, to accurately quantifying SOT, this method allows complete characterization of thermoelectric effects, opening promising avenues for accurate SOT characterization in related systems. In particular, this study corroborates the critical role of naturally oxidized copper interfaced with metallic Cu in the generation of orbital current in Co(2)|Pt(4)|CuOx(3), demonstrating a two-fold increase in damping-like torques compared to a reference sample with an oxidized Al capping layer. These findings offer promising directions for future research on the application aspect of non-equilibrium orbital angular momentum.

Tellegen medium has long been a topic of debate, with its existence being contested over several decades. It was first proposed by Tellegen in 1948 and is characterized by a real-valued cross coupling between electric and magnetic responses, distinguishing it from the well-known chiral medium that has imaginary coupling coefficients. Significantly, Tellegen responses are closely linked to axion dynamics, an extensively studied subject in condensed matter physics. Here, we report the realization of Tellegen metamaterials in the microwave region through a judicious combination of subwavelength metallic resonators, gyromagnetic materials, and permanent magnet discs. We observe the key signature of the Tellegen response, i.e. a Kerr rotation for reflected wave, while the polarization remains the same in the transmission direction. The retrieved effective Tellegen parameter is several orders of magnitude greater than that of natural materials. Our work opens door to a variety of nonreciprocal photonic devices and may provide a platform for studying axion physics.

We theoretically investigate electronic responses to lattice deformation in a ferroaxial system using a tight-binding model on a two-dimensional square lattice and linear response theory. While conventional elastic responses are commonly discussed in terms of symmetric strain, the displacement gradient also contains an antisymmetric component describing a local lattice rotation. Focusing on this rotational degree of freedom, we treat the symmetric strain and antisymmetric local rotation as independent perturbations and incorporate their effects microscopically through deformation-induced modulations of the electronic hopping amplitudes. We find that the local rotation induces characteristic diagonal electric quadrupoles that are distinct from those generated by the symmetric shear strain. The rotation-induced response is dominated by the intraband contribution and increases approximately linearly with the ferroaxial crystal field, vanishing in the absence of ferroaxial order. In contrast, the symmetric-shear-induced response remains finite without ferroaxial order and contains both intraband and interband contributions. These results demonstrate that the antisymmetric local rotation provides a distinct electronic response channel characteristic of the ferroaxial state.

Magnetotactic bacteria (MTB) are a diverse group of microorganisms whose movement can be directed via a magnetic field, which makes them attractive for applications in medicine and microfluidics. One of their key properties is the magnetic moment m, which is challenging to measure experimentally. We perform optical imaging experiments with MSR-1 MTB, and derive both the m statistics and the scaling of m with the MTB size using an explicit and fully automated method to determine m from the MTB trajectories via the U-turn protocol, which measures m based on the U-shaped trajectories exhibited by the MTB in an applied alternating magnetic field. The proposed method is an alternative to the standard U-turn time-based moment calculation and uses the theoretical U-turn shape function we have derived. This directly accounts for the U-turn geometry and determines the moment from the U-turn branch width. We couple this approach with a robust U-turn decomposition algorithm that detects U-turns from MTB tracks regardless of their orientations. We report a linear dependence of m on the size of the bacteria, accounting for the bacteria velocity variations during the U-turns. We also demonstrate that the new U-turn shape-based and the conventional time-based methods produce significantly different results. The proposed method can be used to differentiate between various types of MTB within the same population based on their velocity and magnetic moments, and to precisely characterize the magnetic properties of a culture.

An electro-optic modulator offers the function of modulating the propagation of light in a material with electric field and enables seamless connection between electronics-based computing and photonics-based communication. The search for materials with large electro-optic coefficients and low optical loss is critical to increase the efficiency and minimize the size of electro-optic devices. We present a semi-empirical method to compute the electro-optic coefficients of ferroelectric materials by combining first-principles density-functional theory calculations with Landau-Devonshire phenomenological modeling. We apply the method to study the electro-optic constants, also called Pockels coefficients, of three paradigmatic ferroelectric oxides: BaTiO3, LiNbO3, and LiTaO3. We present their temperature-, frequency- and strain-dependent electro-optic tensors calculated using our method. The predicted electro-optic constants agree with the experimental results, where available, and provide benchmarks for experimental verification.

Polar metals are an underexplored material class combining two properties that are typically incompatible, namely a polar crystal structure and reasonable electrical conductivity. These intriguing materials offer a unique combination of properties, potentially relevant to optoelectronics, catalysis, memory devices, among other applications. The distortive polar metal (DPM) subclass forms through a symmetry-lifting phase transformation into a non-centrosymmetric polar crystal structure. In the process, domains with uniform geometric polar directions form, oftentimes separated by domain boundaries with polarity discontinuities arranged in "charged" head-to-head (H-H) or tail-to-tail (T-T) morphologies. To date, only metallic oxide DPM microstructures have been studied. Here we reveal, in the intermetallic DPM Mn_{5}Al_{8}, different surface interactions and electron transfer reactivity at domain boundaries depending on their H-H or T-T character. Variable surface reactivity suggests localized changes in electronic work functions due to an increase (H-H) or decrease (T-T) in the electronic density of states. These findings suggest that metallic DPMs may offer functionalizable domain boundaries and deserve increased attention, given that they allow tunable chemistries and various thermomechanical processing or transformation protocols. Ultimately, this study proposes unconventional metal physics, propelling the discovery and design of advanced electronic materials and devices.

The Kramers-Kronig relations are a pivotal foundation of linear optics and atomic physics, embedding a physical connection between the real and imaginary components of any causal response function. A mathematically equivalent, but simpler, approach instead utilises the Hilbert transform. In a previous study, the Hilbert transform was applied to absorption spectra in order to infer the sole refractive index of an atomic medium in the absence of an external magnetic field. The presence of a magnetic field causes the medium to become birefringent and dichroic, and therefore it is instead characterised by two refractive indices. In this study, we apply the same Hilbert transform technique to independently measure both refractive indices of a birefringent atomic medium, leading to an indirect measurement of atomic magneto-optical rotation. Key to this measurement is the insight that inputting specific light polarisations into an atomic medium induces absorption associated with only one of the refractive indices. We show this is true in two configurations, commonly referred to in literature as the Faraday and Voigt geometries, which differ by the magnetic field orientation with respect to the light wavevector. For both cases, we measure the two refractive indices independently for a Rb thermal vapour in a 0.6 T magnetic field, finding excellent agreement with theory. This study further emphasises the application of the Hilbert transform to the field of quantum and atomic optics in the linear regime.

We investigate the leading order correction of anomalous magnetic moment (AMM) to the electron in weak magnetic field and find that the magnetic correction is negative and magnetic field dependent, indicating a magnetic catalysis effect for the electron gas. In the laboratory to measure the g-2, the magnitude of the magnetic field B is several T, correspondingly the magnetic correction to the AMM of electron/muon is around 10^{-34}/10^{-42}, therefore the magnetic correction can be safely neglected in current measurement. However, when the magnitude of the magnetic field strength is comparable with the electron mass, the magnetic correction of electron's AMM will become considerable. This general magnetic correction to charged fermion's AMM can be extended to study QCD matter under strong magnetic field.

High magnetic field and low temperature transport is carried out in order to characterize the charge carriers of PtSe_2. In particular, the Shubnikov-de Haas oscillations arising at applied magnetic field strengths gtrsim 4.5,T are found to occur exclusively in plane and emerge at a layer thickness of approx 18,nm, increasing in amplitude and decreasing in frequency for thinner PtSe_2 flakes. Moreover, the quantum transport time, Berry phase, Dingle temperature and cyclotron mass of the charge carriers are ascertained. The emergence of weak antilocalization (WAL) lies in contrast to the presence of magnetic moments from Pt vacancies. An explanation is provided on how WAL and the Kondo effect can be observed within the same material. Detailed information about the charge carriers and transport phenomena in PtSe_2 is obtained, which is relevant for the design of prospective spintronic and orbitronic devices and for the realization of orbital Hall effect-based architectures.

The spin density and Josephson current at equilibrium are studied numerically in a superconductor-normal metal-superconductor (SNS) junction with extrinsic spin-orbit interaction in the N segment. This system preserves structural inversion symmetry. We find that the Josephson current generates the spin Hall effect, resulting in an opposite spin density near the two edges of the N segment. We also find that a Zeeman magnetic field with gradient applied to the N segment generates an anomalous phase shift due to the inverse spin Hall effect, resulting in a diode effect when higher harmonics of the Josephson current are present. These results are consistent with those of a previous theoretical study based on diagrammatic perturbation theory. We find that the diode effect becomes more pronounced when stronger coupling between the N and S segments enhances the higher harmonics.

The Mpemba effect is a thermodynamic anomaly in which a system farther away in temperature from equilibrium thermalizes before one that is initially closer. The effect has been experimentally observed across a wide range of systems, including water, colloids, and trapped ions. It has recently been the focus of numerous studies aimed at understanding its mechanisms and developing multiple applications. Despite extensive work in the field, clearly determining which types of systems exhibit the Mpemba effect remains an open question. To address this, we derive simple necessary conditions on the transition rates for the Mpemba effect in a Markovian 3-level system and show that they can be applied to study the Mpemba effect in an N-level system. Multiple time scales govern thermalization in these systems. This allows the evolution to occur more quickly across larger temperature differences, explaining the Mpemba effect. We apply our protocol to evaluate which types of systems exhibit the Mpemba effect and, in doing so, explain why the Mpemba effect in Markovian systems remains a thermodynamic anomaly. In particular, due to the maximum entropy principle, our conditions allow us to discard the sub-Ohmic and Ohmic spectra. The latter describes a wide range of physical and chemical phenomena, which will not exhibit the Mpemba effect. Moreover, our results provide a clear path to determine the minimal physical requirements for the Mpemba effect, and we apply them to understand its underlying mechanisms better. Finally, our protocol could help identify relevant parameters for experiments, numerical simulations and diverse applications.

Macroscopic EEG fields can be an explicit top-down neocortical mechanism that directly drives bottom-up processes that describe memory, attention, and other neuronal processes. The top-down mechanism considered are macrocolumnar EEG firings in neocortex, as described by a statistical mechanics of neocortical interactions (SMNI), developed as a magnetic vector potential A. The bottom-up process considered are Ca^{2+} waves prominent in synaptic and extracellular processes that are considered to greatly influence neuronal firings. Here, the complimentary effects are considered, i.e., the influence of A on Ca^{2+} momentum, p. The canonical momentum of a charged particle in an electromagnetic field, mathbfΠ = p + q A (SI units), is calculated, where the charge of Ca^{2+} is q = - 2 e, e is the magnitude of the charge of an electron. Calculations demonstrate that macroscopic EEG A can be quite influential on the momentum p of Ca^{2+} ions, in both classical and quantum mechanics. Molecular scales of Ca^{2+} wave dynamics are coupled with A fields developed at macroscopic regional scales measured by coherent neuronal firing activity measured by scalp EEG. The project has three main aspects: fitting A models to EEG data as reported here, building tripartite models to develop A models, and studying long coherence times of Ca^{2+} waves in the presence of A due to coherent neuronal firings measured by scalp EEG. The SMNI model supports a mechanism wherein the p + q A interaction at tripartite synapses, via a dynamic centering mechanism (DCM) to control background synaptic activity, acts to maintain short-term memory (STM) during states of selective attention.

Correlated electron systems are among the centerpieces of modern condensed matter sciences, where many interesting physical phenomena, such as metal-insulator transition and high-Tc superconductivity appear. Recent efforts have been focused on electrostatic doping of such materials to probe the underlying physics without introducing disorder as well as to build field-effect transistors that may complement conventional semiconductor metal-oxide-semiconductor field effect transistor (MOSFET) technology. This review focuses on metal-insulator transition mechanisms in correlated electron materials and three-terminal field effect devices utilizing such correlated oxides as the channel layer. We first describe how electron-disorder interaction, electron-phonon interaction and/or electron correlation in solids could modify the electronic properties of materials and lead to metal-insulator transitions. Then we analyze experimental efforts toward utilizing these transitions in field effect transistors and their underlying principles. It is pointed out that correlated electron systems show promise among these various materials displaying phase transitions for logic technologies. Furthermore, novel phenomena emerging from electronic correlation could enable new functionalities in field effect devices. We then briefly review unconventional electrostatic gating techniques, such as ionic liquid gating and ferroelectric gating, which enables ultra large carrier accumulation density in the correlated materials which could in turn lead to phase transitions. The review concludes with a brief discussion on the prospects and suggestions for future research directions in correlated oxide electronics for information processing.

Light-matter interactions that lead to nonthermal changes in size of the sample constitute a photostrictive effect in many compounds. The photostriction phenomenon was observed in four main groups of materials, ferroelectrics, polar, and non-polar semiconductors, as well as in organic-based materials that are reviewed here. The key mechanisms of photostriction and its dependence on several parameters and perturbations are assessed. The major literature of the photostriction is surveyed, and the review ends with a summary of the proposed technical applications.

We report the anomalous and topological Hall effect of the ferromagnetic Weyl semimetal Mn_5Ge_3. We observe a significant anisotropic anomalous Hall effect (AHE) due to nonzero Berry curvature in the momentum space, such that the anomalous Hall conductivity (AHC) is 965 S/cm for the xy-plane and 233 S/cm for the zx-plane of the single crystal. The band structure calculations predict several Weyl and nodal points span across the momentum space, gapped out under the spin-orbit coupling effect, leading to significant k-space Berry curvature and large AHC. Experimentally, we also demonstrate a sizeable topological Hall effect that is originated by the non-coplanar chiral spin structure due to the competition between the out-of-plane uniaxial magnetocrystalline anisotropy and the dipole-dipole interaction between two Mn sublattices. This study hints at the importance of dipole-dipole interactions in producing the skyrmion lattice in Mn_5Ge_3.

Magnetic cooling has the potential to replace conventional gas compression refrigeration. Materials such as La(Fe,Si)_{13} exhibit a sizeable first-order magnetocaloric effect, and it is possible to tailor the phase transition towards room temperature by Mn-H-doping, resulting in a large temperature range for operation. Within this work, we discuss variations of the electronic and lattice structure in La(Fe,Si)_{13} with increasing Mn content utilizing X-ray magnetic circular dichroism (XMCD) and extended X-ray absorption fine structure spectroscopy (EXAFS). While XMCD shows a decrease of the magnetic polarization at the Fe K edge, low-temperature EXAFS measurements indicate increased positional disorder in the La environment that is otherwise absent for Fe and Mn. First-principles calculations link the positional disorder to an enlarged Mn-Si distance -- explaining the increased positional disorder in the La surrounding.

Initial states of dense matter with nonzero electron chiral imbalance could potentially give rise to strong magnetic fields through chiral plasma instability. Previous work indicated that unless chiral chemical potential is as large as the electron vector chemical potential, the growth of magnetic fields due to the instability is washed out by chirality flipping rate enabled by electron mass. We re-examine this claim in a broader range of parameters and find that at higher temperatures the hierarchy is reversed supporting a growing magnetic field for an initial electron chiral chemical potential much smaller than the electron vector chemical potential. Further, we identify a qualitatively new effect relevant for magnetized hot and dense medium where chiral magnetic effect (CME) sourced by density fluctuation acts as a powerful source of Joule heating. Remarkably, even modest chiral chemical potentials (keV) in such environment can deposit energy densities set by the QCD scale in a relatively short time of the order of a few milliseconds or seconds. We speculate how this mechanism makes CME-driven Joule heating a potentially critical ingredient in the dynamics of turbulent density fluctuation of supernovae and neutron star mergers.

In the photoreceptor compass model, a light-generated, spin-correlated radical pair undergoes singlet-triplet interconversion driven by Zeeman and anisotropic hyperfine interactions, leading to orientation-dependent reaction yields. In this study, we consider simultaneously the spin environment and the boson environment surrounding the radical-pair system and concentrate on the correlated memory effect of the spin bath. In the linear-response limit, the spin bath is mapped to an effective Gaussian environment. The system dynamics and yields under its influence together with the bosonic bath are propagated uniformly using the hierarchical equations of motion (HEOM) or equivalently the dissipaton equations of motion (DEOM) method. The HEOM/DEOM is non-Markovian and non-perturbative, exact for Gaussian environments. Corresponding results of the Markovian Lindblad master equation are also shown for comparison. Numerical demonstrations highlight the non-Markovian memory effect as a crucial ingredient for radical-pair magnetoreception.

The transition from the superconducting to the normal state in a magnetic field was considered as a irreversible thermodynamic process before 1933 because of Joule heating. But all physicists became to consider this transition as reversible after 1933 because of the obvious contradiction of the Meissner effect with the second law of thermodynamics if this transition is considered as a irreversible process. This radical change of the opinion contradicted logic since the dissipation of the kinetic energy of the surface screening current into Joule heat in the normal state cannot depend on how this current appeared in the superconducting state. The inconsistency of the conventional theory of superconductivity, created in the framework of the equilibrium thermodynamics, with Joule heating, on which Jorge Hirsch draws reader's attention, is a consequence of this history. In order to avoid contradiction with the second law of thermodynamics, physicists postulated in the thirties of the last century that the surface screening current is damped without the generation of Joule heat. This postulate contradicts not only logic and the conventional theory of superconductivity but also experimental results.

When a topological insulator is incorporated into a Josephson junction, the system is predicted to reveal the fractional Josephson effect with a 4π-periodic current-phase relation. Here, we report the measurement of a 4π-periodic switching current through an asymmetric SQUID, formed by the higher-order topological insulator WTe_2. Contrary to the established opinion, we show that a high asymmetry in critical current and negligible loop inductance are not sufficient by themselves to reliably measure the current-phase relation. Instead, we find that our measurement is heavily influenced by additional inductances originating from the self-formed PdTe_{x} inside the junction. We therefore develop a method to numerically recover the current-phase relation of the system and find the 1.5,μm long junction to be best described in the short ballistic limit. Our results highlight the complexity of subtle inductance effects that can give rise to misleading topological signatures in transport measurements.

We study the effect of perpendicular magnetic fields on a single-electron system with a strongly time-dependent electrostatic potential. Continuous improvements to the current quantization in these electron pumps are revealed by high-resolution measurements. Simulations show that the sensitivity of tunnel rates to the barrier potential is enhanced, stabilizing particular charge states. Nonadiabatic excitations are also suppressed due to a reduced sensitivity of the Fock-Darwin states to electrostatic potential. The combination of these effects leads to significantly more accurate current quantization.

We report strong unidirectional anisotropy in bulk polycrystalline B20 FeGe measured by ferromagnetic resonance spectroscopy. Bulk and micron-sized samples were produced and analytically characterized. FeGe is a B20 compound with inherent Dzyaloshinskii-Moriya interaction. Lorenz microscopy confirms a skyrmion lattice at 190 ; K in a magnetic field of 150 mT. Ferromagnetic resonance was measured at 276 ; K pm 1 ; K, near the Curie temperature. Two resonance modes were observed, both exhibit a unidirectional anisotropy of K=1153 ; J/m^3 pm 10 ; J/m^3 in the primary, and K=28 ; J/m^3 pm 2 ; J/m^3 in the secondary mode, previously unknown in bulk ferromagnets. Additionally, about 25 standing spin wave modes are observed inside a micron-sized FeGe wedge, measured at room temperature (sim ; 293 K). These modes also exhibit unidirectional anisotropy.

We discuss the effect of a strong magnetic field on the chemical freezeout points in the ultrarelativistic heavy-ion collision. As a result of the inverse magnetic catalysis or the magnetic inhibition, the crossover onset to hot and dense matter out of quarks and gluons should be shifted to a lower temperature. To quantify this shift we employ the hadron resonance gas model and an empirical condition for the chemical freezeout. We point out that the charged particle abundances are significantly affected by the magnetic field so that the electric charge fluctuation is largely enhanced especially at high baryon density. The charge conservation partially cancels the enhancement but our calculation shows that the electric charge fluctuation and the charge chemical potential could serve as a magnetometer. We find that the fluctuation exhibits a crossover behavior rapidly increased for eB >~ (0.4GeV)^2, while the charge chemical potential has better sensitivity to the magnetic field.

Perovskite ABO_3 oxides display an amazing variety of phenomena that can be altered by subtle changes in the chemistry and internal structure, making them a favorite class of materials to explore the rational design of novel properties. Here we highlight a recent advance in which rotations of the BO_6 octahedra give rise to a novel form of ferroelectricity -- hybrid improper ferroelectricity. Octahedral rotations also strongly influence other structural, magnetic, orbital, and electronic degrees of freedom in perovskites and related materials. Octahedral rotation-driven ferroelectricity consequently has the potential to robustly control emergent phenomena with an applied electric field. The concept of `functional' octahedral rotations is introduced and the challenges for materials chemistry and the possibilities for new rotation-driven phenomena in multifunctional materials are explored.

The emergence of two-dimensional (2D) materials has attracted a great deal of attention due to their fascinating physical properties and potential applications for future nanoelectronic devices. Since the first isolation of graphene, a Dirac material, a large family of new functional 2D materials have been discovered and characterized, including insulating 2D boron nitride, semiconducting 2D transition metal dichalcogenides and black phosphorus, and superconducting 2D bismuth strontium calcium copper oxide, molybdenum disulphide and niobium selenide, etc. Here, we report the identification of ferromagnetic thin flakes of Cr2Ge2Te6 (CGT) with thickness down to a few nanometers, which provides a very important piece to the van der Waals structures consisting of various 2D materials. We further demonstrate the giant modulation of the channel resistance of 2D CGT devices via electric field effect. Our results illustrate the gate voltage tunability of 2D CGT and the potential of CGT, a ferromagnetic 2D material, as a new functional quantum material for applications in future nanoelectronics and spintronics.

This review presents recent breakthroughs in the realm of nonlinear Hall effects, emphasizing central theoretical foundations and recent experimental progress. We elucidate the quantum origin of the second-order Hall response, focusing on the Berry curvature dipole, which may arise in inversion symmetry broken systems. The theoretical framework also reveals the impact of disorder scattering effects on the nonlinear response. We further discuss the possibility of obtaining nonlinear Hall responses beyond the second order. We examine symmetry-based indicators essential for the manifestation of nonlinear Hall effects in time-reversal symmetric crystals, setting the stage for a detailed exploration of theoretical models and candidate materials predicted to exhibit sizable and tunable Berry curvature dipole. We summarize groundbreaking experimental reports on measuring both intrinsic and extrinsic nonlinear Hall effects across diverse material classes. Finally, we highlight some of the other intriguing nonlinear effects, including nonlinear planar Hall, nonlinear anomalous Hall, and nonlinear spin and valley Hall effects. We conclude with an outlook on pivotal open questions and challenges, marking the trajectory of this rapidly evolving field.

Controlling magnetic phases and properties through composition and external conditions is central to the development of magnetic materials. Atomistic foundation models offer a route to predicting such behaviour across diverse materials, but magnetic materials remain challenging because their atomic structure and local moments are strongly coupled, while temperature and disorder drive magnetic moments into non-collinear states with evolving orientations and magnitudes. Broadly pretrained atomistic models still sample only limited magnetic diversity, while finite-temperature descriptions of coupled lattice and magnetic fluctuations remain largely material-specific. Here we introduce MagPT, pretrained across 48 elements on 912,492 spin-lattice configurations spanning structural, orientational and longitudinal magnetic fluctuations over 0 sim 1,000 K and 0 sim 10 GPa. By treating species, atomic positions and vector moments together, MagPT distinguishes magnetic states that share the same atomic structure but differ in spin configuration and energy. It captures magnetic behaviour across composition, temperature and length scales, from Slater-Pauling-type composition-magnetism relations in transition-metal alloys and finite-temperature phase evolution in elemental ferromagnets and magnetic shape-memory Heusler alloys, to emergent long-wavelength non-collinear spin textures in chiral magnets and local chemistry-magnetism coupling in high-entropy alloys. MagPT moves atomistic studies of magnetic materials beyond material-specific approaches, establishing a general framework for exploring and designing magnetic matter across diverse chemistries and conditions.

The Orbital Hall effect, which originates from materials with weak spin-orbit coupling, has attracted considerable interest for spin-orbitronic applications. Here, we demonstrate the inverse effect of the orbital Hall effect and observe orbitronic terahertz emission in the Ti and Mn materials. Through spin-orbit transition in the ferromagnetic layer, the generated orbital current can be converted to charge current in the Ti and Mn layers via the inverse orbital Hall effect. Furthermore, the inserted W layer provides an additional conversion of the orbital-charge current in the Ti and Mn layers, significantly enhancing the orbitronic terahertz emission. Moreover, the orbitronic terahertz emission can be manipulated by cooperating with the inverse orbital Hall effect and the inverse spin Hall effect in the different sample configurations. Our results not only discover the physical mechanism of condensed matter physics but also pave the way for designing promising spin-orbitronic devices and terahertz emitters.

In complex oxide materials, changes in electronic properties are often associated with changes in crystal structure, raising the question of the relative roles of the electronic and lattice effects in driving the metal-insulator transition. This paper presents a combined theoretical and experimental analysis of the dependence of the metal-insulator transition of NdNiO_3 on crystal structure, specifically comparing properties of bulk materials to one and two layer samples of NdNiO_3 grown between multiple electronically inert NdAlO_3 counterlayers in a superlattice. The comparison amplifies and validates a theoretical approach developed in previous papers and disentangles the electronic and lattice contributions, through an independent variation of each. In bulk NdNiO_3 the correlations are not strong enough to drive a metal-insulator transition by themselves: a lattice distortion is required. Ultra-thin films exhibit two additional electronic effects and one lattice-related effect. The electronic effects are quantum confinement, leading to dimensional reduction of the electronic Hamiltonian, and an increase in electronic bandwidth due to counterlayer induced bond angle changes. We find that the confinement effect is much more important. The lattice effect is an increase in stiffness due to the cost of propagation of the lattice disproportionation into the confining material.

It stands to reason that the amount and the quality of data is of key importance for setting up accurate AI-driven models. Among others, a fundamental aspect to consider is the bias introduced during sample selection in database generation. This is particularly relevant when a model is trained on a specialized dataset to predict a property of interest, and then applied to forecast the same property over samples having a completely different genesis. Indeed, the resulting biased model will likely produce unreliable predictions for many of those out-of-the-box samples. Neglecting such an aspect may hinder the AI-based discovery process, even when high quality, sufficiently large and highly reputable data sources are available. In this regard, with superconducting and thermoelectric materials as two prototypical case studies in the field of energy material discovery, we present and validate a new method (based on a classification strategy) capable of detecting, quantifying and circumventing the presence of cross-domain data bias.

Advances in scaling down heterostructures and having an improved interface quality together with atomically-thin two-dimensional materials suggest a novel approach to systematically design materials. A given material can be transformed through proximity effects whereby it acquires properties of its neighbors, for example, becoming superconducting, magnetic, topologically nontrivial, or with an enhanced spin-orbit coupling. Such proximity effects not only complement the conventional methods of designing materials by doping or functionalization, but can also overcome their various limitations. In proximitized materials it is possible to realize properties that are not present in any constituent region of the considered heterostructure. While the focus is on magnetic and spin-orbit proximity effects with their applications in spintronics, the outlined principles provide also a broader framework for employing other proximity effects to tailor materials and realize novel phenomena.

Molecular ferroelectric materials have attracted widespread attention due to their abundant chemical diversity, structural tunability, low synthesis temperature, and high flexibility. Meanwhile, the integration of molecular ferroelectric materials and Si is still challenging, while the fundamental understanding of the ferroelectric switching process is still lacking. Herein, we have successfully synthesized the imidazole perchlorate (ImClO4) single crystals and a series of high-quality highly-oriented thin films on a Si substrate. A high inverse piezoelectric coefficient (55.7 pm/V) is demonstrated for the thin films. Two types of domain bands can be observed (in the size of a few microns): type-I band tilts ~60{\deg} with respect to the horizontal axis, while the type-II band is perpendicular to the horizontal axis. Most of the domain walls (DWs) are 180{\deg} DWs for the two bands, while some 109{\deg} DWs can also be observed. Interestingly, the DWs in type-I band are curved, charged domain walls; while the 180{\deg} DWs in type-II band are straight, noncharged domain walls. After applying +20 V for 5 s through a PFM tip, the 180{\deg} DWs in type-I band shrink first, then disconnect from the band boundary, forming a needle-like domain with a size of ~100 nm. The needle-like domain will extend toward the band boundary after an inverse bias is applied (-20 V), and expand along the band boundary after touching the boundary. Whereas for the type-II domain band, the 180{\deg} DWs are more mobile than the 109{\deg} domain walls, which displaces ~500 nm after applying +20 V. While such displacement is much shorter after the application of a negative bias for the same duration, starting from the positively poled sample. We hope to spur further interest in the on-chip design of the molecular ferroelectrics based electronic devices.

Significant progress on parameter-free calculations of carrier mobilities in real materials has been made during the past decade; however, the role of various approximations remains unclear and a unified methodology is lacking. Here, we present and analyse a comprehensive and efficient approach to compute the intrinsic, phonon-limited drift and Hall carrier mobilities of semiconductors, within the framework of the first-principles Boltzmann transport equation. The methodology exploits a novel approach for estimating quadrupole tensors and including them in the electron-phonon interactions, and capitalises on a rigorous and efficient procedure for numerical convergence. The accuracy reached in this work allows to assess common approximations, including the role of exchange and correlation functionals, spin-orbit coupling, pseudopotentials, Wannier interpolation, Brillouin-zone sampling, dipole and quadrupole corrections, and the relaxation-time approximation. A detailed analysis is showcased on ten prototypical semiconductors, namely diamond, silicon, GaAs, 3C-SiC, AlP, GaP, c-BN, AlAs, AlSb, and SrO. By comparing this extensive dataset with available experimental data, we explore the intrinsic nature of phonon-limited carrier transport and magnetotransport phenomena in these compounds. We find that the most accurate calculations predict Hall mobilities up to a factor of two larger than experimental data; this could point to promising experimental improvements in the samples quality, or to the limitations of density-function theory in predicting the carrier effective masses and overscreening the electron-phonon matrix elements. By setting tight standards for reliability and reproducibility, the present work aims to facilitate validation and verification of data and software towards predictive calculations of transport phenomena in semiconductors.

Comprehensive study using DC transport, specific heat, magnetization, and two-coil mutual inductance measurements unveils an understanding of three temperature regimes in SmB_6: (i) T geq T^{*} (sim66K), (ii) T_g (sim40 K) leq T < T^{*}, and (iii) T < T_g. Onset of Kondo breakdown below T^{*} releases disorder-driven magnetic fluctuations, which splits the bulk (sim116K) and surface Kondo temperature (T_k^{s} approx 7 K). Below T_g, as magnetic fluctuations subside, surface Kondo screening revives, stabilizing the topological surface state and generating an in-gap feature (sim2.2 meV) across which Dirac-like carriers are excited. Nyquist impedance analysis reveals a crossover from purely capacitive to capacitive-inductive behavior, signalling a disorder-driven two-fluid phase of heavy quasiparticles and light, high-mobility carriers below T_g. We identify a characteristic length scale, L_{ν_0}(T), associated with the high-mobility phase, exhibiting an almost divergent trend below T_k^{s}. These findings underscore the complex nature of the surface conducting state in SmB_6.

The NMR measurements performed on a single orthorhombic crystal of superconducting ferromagnet UCoGe (Y.Ihara et al, Phys. Rev. Lett. v.105, 206403 (2010)) demonstrate strongly anisotropic magnetic properties of this material. The presented calculations allow to establish the dependence of longitudinal spin-lattice relaxation rate from temperature and magnetic field. The value 1/T_1T in field perpendicular to spontaneous magnetisation directed along c-axis has maximum in vicinity of Curie temperature whereas it does not reveal similar behaviour in field parallel to the direction of spontaneous magnetisation. Also there was shown that the longitudinal spin-lattice relaxation rate is strongly field dependent when the field directed in b-crystallographic direction but field independent if magnetic field is oriented along a-axis.

Within the paradigm of metamaterials and metasurfaces, electromagnetic properties of composite materials can be engineered by shaping or modulating their constituents, so-called meta-atoms. Synthesis and analysis of complex-shape meta-atoms with general polarization properties is a challenging task. In this paper, we demonstrate that the most general response can be conceptually decomposed into a set of basic, fundamental polarization phenomena, which enables immediate all-direction characterization of electromagnetic properties of arbitrary linear metamaterials and metasurfaces. The proposed platform of modular characterization (called "materiatronics") is tested on several examples of bianisotropic and nonreciprocal meta-atoms. As a demonstration of the potential of the modular analysis, we use it to design a single-layer metasurface of vanishing thickness with unitary circular dichroism. The analysis approach developed in this paper is supported by a ready-to-use computational code and can be further extended to meta-atoms engineered for other types of wave interactions, such as acoustics and mechanics.

The finite-temperature magnetic properties of Fe_xPd_{1-x} and Co_xPt_{1-x} alloys have been investigated. It is shown that the temperature-dependent magnetic behaviour of alloys, composed of originally magnetic and non-magnetic elements, cannot be described properly unless the coupling between magnetic moments at magnetic atoms (Fe,Co) mediated through the interactions with induced magnetic moments of non-magnetic atoms (Pd,Pt) is included. A scheme for the calculation of the Curie temperature (T_C) for this type of systems is presented which is based on the extended Heisenberg Hamiltonian with the appropriate exchange parameters J_{ij} obtained from {\em ab-initio} electronic structure calculations. Within the present study the KKR Green's function method has been used to calculate the J_{ij} parameters. A comparison of the obtained Curie temperatures for Fe_xPd_{1-x} and Co_xPt_{1-x} alloys with experimental data shows rather good agreement.

The transition of an impulsively excited kink oscillation of a solar coronal loop to an oscillation with a stationary amplitude, i.e., the damping pattern, is determined using the low-dimensional self-oscillation model. In the model, the decayless kink oscillations are sustained by the interaction of the oscillating loop with an external quasi-steady flow. The analytical solution is based on the assumption that the combined effect of the effective dissipation, for example, by resonant absorption, and interaction with an external flow, is weak. The effect is characterised by a dimensionless coupling parameter. The damping pattern is found to depend upon the initial amplitude and the coupling parameter. The approximate expression shows a good agreement with a numerical solution of the self-oscillation equation. The plausibility of the established damping pattern is demonstrated by an observational example. Notably, the damping pattern is not exponential, and the characteristic decay time is different from the time determined by the traditionally used exponential damping fit. Implications of this finding for seismology of the solar coronal plasmas are discussed. In particular, it is suggested that a very rapid, in less than the oscillation period, decay of the oscillation to the stationary level, achieved for larger values of the coupling parameter, can explain the relative rareness of the kink oscillation events.

Resistivity, magnetization and microscopic ^{75}As nuclear magnetic resonance (NMR) measurements in the antiferromagnetically ordered state of the iron-based superconductor parent material CaFe_2As_2 exhibit anomalous features that are consistent with the collective freezing of domain walls. Below T^*approx 10 K, the resistivity exhibits a peak and downturn, the bulk magnetization exhibits a sharp increase, and ^{75}As NMR measurements reveal the presence of slow fluctuations of the hyperfine field. These features in both the charge and spin response are strongly field dependent, are fully suppressed by H^*approx 15 T, and suggest the presence of filamentary superconductivity nucleated at the antiphase domain walls in this material.

We report a quasi-one-dimensional S = 1 spin chain compound BaNiTe2O7. This magnetic system has been investigated by magnetic susceptibility, specific heat, and neutron powder diffraction. These results indicate that BaNiTe2O7 develops a short-range magnetic correlation around T ~ 22 K. With further cooling, an antiferromagnetic phase transition is observed at TN ~ 5.4 K. Neutron powder diffraction revealed antiferromagnetic noncollinear order with a commensurate propagation vector k = (1/2, 1, 0). The refined magnetic moment size of Ni2+ at 1.5 K is 1.84{\mu}B, and its noncollinear spin texture is confirmed by first-principles calculations. Inelastic neutron-scattering results and density functional theory calculations confirmed the quasi-one-dimensional nature of the spin systems.

Permanent magnets draw their properties from a complex interplay of chemical composition and phase, each with their associated intrinsic magnetic properties. Gaining an understanding of these interactions is the key to deciphering the origins of a permanent magnets' magnetic performance and facilitate the engineering of much improved-performing magnets. Here, we use advanced multiscale microscopy and microanalysis on a bulk Sm2(Co,Fe,Cu,Zr)17 pinning-type high-performance magnet with outstanding thermal and chemical stability. Comparison of the microstructure in regions of different composition, we demonstrate that the pinning of magnetic domains, imaged by nanoscale magnetic induction mapping, is controlled by the composition and atomic arrangement of copper. This is confirmed by micromagnetic simulations. Contrary to the belief that grain boundaries are "weak links" in magnetic materials, we demonstrate grain boundaries undergo magnetization reversal at relatively low fields (0.1-0.3 T), but this remains confined to these regions and does not significantly impact the magnet's coercivity. Our results showcase that it is the optimal microstructure within the grain itself that is crucial for achieving the desired magnetic properties.

We have systematically investigated the grain boundary (GB) angle dependence of transport properties for NdFeAs(O,F) fabricated on [001]-tilt symmetric MgO bicrystal substrates. In our previous study, NdFeAs(O,F) bicrystal films showed a weak-link behaviour even at a GB angle of 6°. However, this was caused by an extrinsic effect originating from the damage to both NdFeAs(O,F) and MgO substrate by excess F-diffusion along the grain boundary. To investigate the intrinsic nature of grain boundaries, we minimized the damage to NdFeAs(O,F) and MgO by reducing the deposition temperature of NdOF over-layer needed for F-doping. The resultant NdFeAs(O,F) bicrystal films have a critical angle of 8.5°, above which Jc starts to decrease exponentially. This critical angle is almost the same as those of other Fe-based superconductors.

It was previously believed that the Bloch electronic states of non-magnetic materials with inversion symmetry cannot have finite spin polarizations. However, since the seminal work by Zhang et al. [Nat. Phys. 10, 387-393 (2014)] on local spin polarizations of Bloch states in non-magnetic, centrosymmetric materials, the scope of spintronics has been significantly broadened. Here, we show, using a framework that is universally applicable independent of whether hidden spin polarizations are small (e.g., diamond, Si, Ge, and GaAs) or large (e.g., MoS2 and WSe2), that the corresponding quantity arising from orbital - instead of spin - degrees of freedom, the hidden orbital polarization, is (i) much more abundant in nature since it exists even without spin-orbit coupling and (ii) more fundamental since the interband matrix elements of the site-dependent orbital angular momentum operator determines the hidden spin polarization. We predict that the hidden spin polarization of transition metal dichalcogenides is reduced significantly upon compression. We suggest experimental signatures of hidden orbital polarization from photoemission spectroscopies and demonstrate that the current-induced hidden orbital polarization may play a far more important role than its spin counterpart in antiferromagnetic information technology by calculating the current-driven antiferromagnetism in compressed silicon.

Trapped fields of over 20 T are, in principle, achievable in bulk, single-grain high temperature cuprate superconductors. The principle barriers to realizing such performance are, firstly, the large tensile stresses that develop during the magnetization of such trapped-field magnets as a result of the Lorentz force, which lead to brittle fracture of these ceramic-like materials at high fields and, secondly, catastrophic thermal instabilities as a result of flux movement during magnetization. Moreover, for a batch of samples nominally fabricated identically, the statistical nature of the failure mechanism means the best performance (i.e. trapped fields of over 17 T) cannot be attained reliably. The magnetization process, particularly to higher fields, also often damages the samples such that they cannot repeatedly trap high fields following subsequent magnetization. In this study, we report the sequential trapping of magnetic fields of ~ 17 T, achieving 16.8 T at 26 K initially and 17.6 T at 22.5 K subsequently, in a stack of two Ag-doped GdBa2Cu3O7-δ bulk superconductor composites of diameter 24 mm reinforced with (1) stainless-steel laminations, and (2) shrink-fit stainless steel rings. A trapped field of 17.6 T is, in fact, comparable with the highest trapped fields reported to date for bulk superconducting magnets of any mechanical and chemical composition, and this was achieved using the first composite stack to be fabricated by this technique.

This study examines the performance of finite spin quantum batteries (QBs) using Heisenberg spin models with Dzyaloshinsky-Moriya (DM) and Kaplan--Shekhtman--Entin-Wohlman--Aharony (KSEA) interactions. The QBs are modeled as interacting quantum spins in local inhomogeneous magnetic fields, inducing variable Zeeman splitting. We derive analytical expressions for the maximal extractable work, ergotropy and the capacity of QBs, as recently examined by Yang et al. [Phys. Rev. Lett. 131, 030402 (2023)]. These quantities are analytically linked through certain quantum correlations, as posited in the aforementioned study. Different Heisenberg spin chain models exhibit distinct behaviors under varying conditions, emphasizing the importance of model selection for optimizing QB performance. In antiferromagnetic (AFM) systems, maximum ergotropy occurs with a Zeeman splitting field applied to either spin, while ferromagnetic (FM) systems benefit from a uniform Zeeman field. Temperature significantly impacts QB performance, with ergotropy in the AFM case being generally more robust against temperature increases compared to the FM case. Incorporating DM and KSEA couplings can significantly enhance the capacity and ergotropy extraction of QBs. However, there exists a threshold beyond which additional increases in these interactions cause a sharp decline in capacity and ergotropy. This behavior is influenced by temperature and quantum coherence, which signal the occurrence of a sudden phase transition. The resource theory of quantum coherence proposed by Baumgratz et al. [Phys. Rev. Lett. 113, 140401 (2014)] plays a crucial role in enhancing ergotropy and capacity. However, ergotropy is limited by both the system's capacity and the amount of coherence. These findings support the theoretical framework of spin-based QBs and may benefit future research on quantum energy storage devices.

Ultrafast electron microscopy (UEM) has found widespread applications in physics, chemistry, and materials science, enabling real-space imaging of dynamics on ultrafast timescales. Recent advances have pushed the temporal resolution of UEM into the attosecond regime, enabling the attomicroscopy technique to directly visualize electron motion. In this work, we extend the capabilities of this powerful imaging tool to investigate ultrafast electron dynamics in a biological system by imaging and controlling light induced electronic and chemical changes in the conductive network of multicellular cable bacteria. Using electron energy loss spectroscopy (EELS), we first observed a laser induced increase in {\pi}-electron density, accompanied by spectral peak broadening and a blueshift features indicative of enhanced conductivity and structural modification. We also traced the effect of ultrafast laser pumping on bulk plasmon electron oscillations by monitoring changes in the plasmon like resonance peak. Additionally, we visualized laser induced chemical structural changes in cable bacteria in real space. The imaging results revealed carbon enrichment alongside a depletion of nitrogen and oxygen, highlighting the controllability of chemical dynamics. Moreover, time resolved EELS measurements further revealed a picosecond scale decay and recovery of both {\pi}-electron and plasmonic features, attributed to electron phonon coupling. In addition to shedding light on the mechanism of electron motion in cable bacteria, these findings demonstrate ultrafast modulation and switching of conductivity, underscoring their potential as bio-optoelectronic components operating on ultrafast timescales.

The Sun's outer atmosphere, the corona, is maintained at mega-Kelvin temperatures and fills the heliosphere with a supersonic outflowing wind. The dissipation of magnetic waves and direct electric currents are likely to be the most significant processes for heating the corona, but a lively debate exists on their relative roles. Here, we suggest that the two are often intrinsically linked, since magnetic waves may trigger current dissipation, and impulsive reconnection can launch magnetic waves. We present a study of the first of these processes by using a 2D physics-based numerical simulation using the Adaptive Mesh Refined (AMR) Versatile Advection Code (VAC). Magnetic waves such as fast magnetoacoustic waves are often observed to propagate in the large-scale corona and interact with local magnetic structures. The present numerical simulations show how the propagation of magnetic disturbances towards a null point or separator can lead to the accumulation of the electric currents. Lorentz forces can laterally push and vertically stretch the magnetic fields, forming a current sheet with a strong magnetic-field gradient. The magnetic field lines then break and reconnect, and so contribute towards coronal heating. Numerical results are presented that support these ideas and support the concept of a symbiosis between waves and reconnection in heating the solar corona.

The amplitude of ground state superconducting energy gap Δ(0) and relative jump in electronic specific heat at the transition temperature, ΔC{/}γT_c, are primary fundamental parameters of any superconductor. There are several well-established techniques to measure these values for bulk samples. However, there is limited number of techniques which can be applied to measure these parameters in atomically thin superconductors. Here we proposed a new approach to extract Δ(0) and ΔC{/}γT_c in atomically thin superconductors by utilizing perpendicular, Bc2,perp(T) (when magnetic field is applied in perpendicular direction to the film surface), and parallel, Bc2,||(T) (when magnetic field is applied in parallel direction to the film surface), upper critical field data. Deduced parameters for few layers thick Al, Sn, NbSe2, MoS2, magic angle twisted trilayer graphene (MATTG), and WTe2 are well matched values expected for strong- and moderately strong-coupled electron-phonon mediated superconductors. Observed, in many atomically thin superconductors, an enhancement of Bc2,||(0) above the Pauli-Clogston-Chandrasekhar limiting field (i.e., magnetic field required to break the Cooper pair) is explained based on the sample geometry, without an assumption that some exotic pairing mechanism, for instance, Ising-type, is emergent in these materials.

Dielectric materials, with high tunability at microwave frequencies, are key components in the design of microwave communication systems. Dense Ba0.6Sr0.4TiO3 (BST) ceramics, with different grain sizes, were prepared in order to optimise the dielectric tunability via polar nano cluster effects. Dielectric permittivity and loss measurements were carried at both high and low frequencies and were supported by results from X-ray powder diffraction, scanning and transmission electron microscopies, Raman spectroscopy and piezoresponse force microscopy. The concentration of polar nano clusters, whose sizes are found to be in the range 20 to 50 nm, and the dielectric tunability increase with increasing grain size. A novel method for measurement of the microwave tunability in bulk dielectrics is presented. The highest tunability of 32% is achieved in ceramics with an average grain size of 10 um. The tunability of BST ceramics with applied DC field is demonstrated in a prototype small resonant antenna.

Based on a time-dependent Ginzburg-Landau system of equations and finite element modeling, we present novel results related with the physics of phase-slippage in superconducting wires surrounded by a non-superconductive environment. These results are obtained within our previously reported approach related to superconducting rings and superconductive gravitational wave detector transducers. It is shown that the phase-slip centers (PSCs) can be effective in originating not only positive but also negative thermal fluxes. With an appropriate design utilizing thermal diodes, PSCs can serve as cryocooling engines. Operating at Tsim 1 K cryostat cold-finger, they can achieve sub-Kelvin temperatures without using ^3He.

The paper proposes a generalization of the fully implicit energy- and charge-conserving electromagnetic particle-in-cell method to the case where the lightest type of plasma particle (electrons) is described in the drift-kinetic approximation. This allows us to remove the very strict time step limitation of this method requiring to resolve the gyrorotation of electrons. Since the drift-kinetic model is only applicable to light particles whose contribution to plasma polarization is small, this model can be further simplified by neglecting the electron polarization drift and including in Maxwell's equations, in addition to the current of gyrocenters, only the magnetization current. In order for such a hybrid model to retain conservative properties in finite-difference form, a method of self-consistent interpolation of nabla B in the mirror force from grid to particle and the magnetization vector from particle to grid is proposed. Unlike existing drift-kinetic models, this model is not limited to considering small perturbations near a given equilibrium, and therefore allows one to study the formation of plasma equilibria in regimes with a finite ratio of plasma to magnetic field pressure. Testing of the parallel code implemented in C++ using the PETSc library confirmed the fulfillment of the finite-difference laws of energy and charge conservation, as well as the ability of the model (in the drift-kinetic version for all types of particles) to correctly reproduce the diamagnetic effect and longitudinal ion-acoustic wave.

We investigate Josephson arrays consisting of a dice-lattice network of superconducting weak links surrounding rhombic plaquettes of proximitized semiconductor. Josephson coupling of the weak links and electron density in the plaquettes are independently controlled by separate electrostatic gates. Applied magnetic flux results in an intricate pattern of switching currents associated with frustration, f. For depleted plaquettes, the switching current is nearly periodic in f, expected for a phase-only description, while occupied plaquettes yield a decreasing envelope of switching currents with increasing f. A model of flux dependence based on ballistic small-area junctions and diffusive large-area plaquettes yields excellent agreement with experiment.

In chemistry and biochemistry, chirality represents the structural asymmetry characterized by non-superimposable mirror images for a material like DNA. In physics, however, chirality commonly refers to the spin-momentum locking of a particle or quasiparticle in the momentum space. While seemingly disconnected, structural chirality in molecules and crystals can drive electronic chirality through orbital-momentum locking, i.e. chirality can be transferred from the atomic geometry to electronic orbitals. Electronic chirality provides an insightful understanding of the chirality-induced spin selectivity (CISS), in which electrons exhibit salient spin polarization after going through a chiral material, and electric magnetochiral anisotropy (EMCA), which is characterized by the diode-like transport. It further gives rise to new phenomena, such as anomalous circularly polarized light emission (ACPLE), in which the light handedness relies on the emission direction. These chirality-driven effects will generate broad impacts in fundamental science and technology applications in spintronics, optoelectronics, and biochemistry.

Extracting the London penetration depth, λ(T), from the measured magnetic susceptibility, χ(T), of a superconducting platelet in a perpendicular magnetic field requires knowing the function χ(λ) computed for the actual sample geometry. Thin films are increasingly important in quantum computing and superconducting electronics, most of which operate at ultra-low excitation fields in the vortex-free regime. Understanding their electromagnetic response in the Meissner--London (finite-λ, no vortices) state is therefore essential for extracting intrinsic properties such as the London penetration depth and superfluid phase stiffness. While numerous prior works have addressed different aspects of this problem, here we focus on providing an analytical semi-empirical representation of χ(λ) based on the 2D sheet-current model and establishing the limits of its applicability using two independent full 3D numerical solutions: finite-element modeling and a volume-current integral equation. As a result, we provide χ(λ) for a disc of radius a and thickness d in closed form, valid for all λ and for aspect ratios δequiv d/(2a)le0.05, and accurate to 0.1%. The two-dimensional sheet description with Pearl length Λ=2λ^2/d is adequate for δlesssim10^{-4} and λgtrsim 4d. Thicker films require the full closed form, which includes the three-dimensional corrections. Using the same numerical analysis, we provide an empirical formula that maps rectangular samples---the geometry most commonly used in experiments---onto a disc with an ``effective radius'' for subsequent calculation of χ(λ), and formulate a complete calibration protocol for whole-sample susceptibility measurements.

We investigate in more detail the holographic model of a superconductor recently found by Hartnoll, Herzog, and Horowitz [Phys. Rev. Lett. 101, 031601], which is constructed from a condensate of a charged scalar field in AdS_4-Schwarzschild background. By analytically studying the perturbation of the gravitational system near the critical temperature T_c, we obtain the superconducting coherence length proportional to 1/1-T/T_c via AdS/CFT correspondence. By adding a small external homogeneous magnetic field to the system, we find that a stationary diamagnetic current proportional to the square of the order parameter is induced by the magnetic field. These results agree with Ginzburg-Landau theory and strongly support the idea that a superconductor can be described by a charged scalar field on a black hole via AdS/CFT duality.

The twist-grain-boundary (TGB) phases, characterized by a periodic, helical arrangement of blocks made of polar smectic phases, SmAF and SmCF, have been discovered. They have been observed for rod-like molecules with a strong longitudinal dipole moment, featuring an (S)-2-methylbutyl end group having only weak twisting power, and emerge below the antiferroelectric SmAAF phase, where the lamellar structure is already well established. It is suggested that the structure is governed by electrostatic interactions amplified by weak chiral forces, in striking contrast to the mechanism of TGB phase formation found in non-polar materials. The TGB phases exhibit light selective reflection in the visible range, while the value of electric polarization confirms an almost perfectly ordered dipole alignment.

As scanning tunneling microscopy is pushed towards fast local dynamics, a quantitative understanding of tunnel junctions under the influence of a fast AC driving signal is required, especially at the ultra-low temperatures relevant to spin dynamics and correlated electron states. We subject a superconductor-insulator-superconductor junction to a microwave signal from an antenna mounted in situ and examine the DC response of the contact to this driving signal. Quasi-particle tunneling and the Josephson effect can be interpreted in the framework of Tien-Gordon theory. The situation is more complex when it comes to higher order effects such as multiple Andreev reflections. Microwave assisted tunneling unravel these complex processes, providing deeper insights into tunneling than are available in a pure DC measurement.

Materials combining both a high refractive index and a wide band gap are of great interest for optoelectronic and sensor applications. However, these two properties are typically described by an inverse correlation with high refractive index appearing in small gap materials and vice-versa. Here, we conduct a first-principles high-throughput study on more than 4000 semiconductors (with a special focus on oxides). Our data confirm the general inverse trend between refractive index and band gap but interesting outliers are also identified. The data are then analyzed through a simple model involving two main descriptors: the average optical gap and the effective frequency. The former can be determined directly from the electronic structure of the compounds, but the latter cannot. This calls for further analysis in order to obtain a predictive model. Nonetheless, it turns out that the negative effect of a large band gap on the refractive index can counterbalanced in two ways: (i) by limiting the difference between the direct band gap and the average optical gap which can be realized by a narrow distribution in energy of the optical transitions and (ii) by increasing the effective frequency which can be achieved through either a high number of transitions from the top of the valence band to the bottom of the conduction or a high average probability for these transitions. Focusing on oxides, we use our data to investigate how the chemistry influences this inverse relationship and rationalize why certain classes of materials would perform better. Our findings can be used to search for new compounds in many optical applications both in the linear and non-linear regime (waveguides, optical modulators, laser, frequency converter, etc.).

In geometrically frustrated magnetic systems, weak interactions or slight changes to the structure can tip the delicate balance of exchange interactions, sending the system into a different ground state. Brochantite, Cu_4SO_4(OH)_6, has a copper sublattice composed of distorted triangles, making it a likely host for frustrated magnetism, but exhibits stacking disorder. The lack of synthetic single crystals has limited research on the magnetism in brochantite to powders and natural mineral crystals. We grew crystals which we find to be a new polytype with a tendency toward ABAC stacking and some anion disorder, alongside the expected stacking disorder. Comparison to previous results on natural mineral specimens suggests that cation disorder is more deleterious to the magnetism than anion and stacking disorder. Our specific heat data suggest a double transition on cooling into the magnetically ordered state.

Electron-electron (e-e) and electron-phonon (e-ph) interactions are challenging to describe in correlated materials, where their joint effects govern unconventional transport, phase transitions, and superconductivity. Here we combine first-principles e-ph calculations with dynamical mean field theory (DMFT) as a step toward a unified description of e-e and e-ph interactions in correlated materials. We compute the e-ph self-energy using the DMFT electron Green's function, and combine it with the e-e self-energy from DMFT to obtain a Green's function including both interactions. This approach captures the renormalization of quasiparticle dispersion and spectral weight on equal footing. Using our method, we study the e-ph and e-e contributions to the resistivity and spectral functions in the correlated metal Sr_2RuO_4. In this material, our results show that e-e interactions dominate transport and spectral broadening in the temperature range we study (50-310~K), while e-ph interactions are relatively weak and account for only sim10\% of the experimental resistivity. We also compute effective scattering rates, and find that the e-e interactions result in scattering several times greater than the Planckian value k_BT, whereas e-ph interactions are associated with scattering rates lower than k_BT. Our work demonstrates a first-principles approach to combine electron dynamical correlations from DMFT with e-ph interactions in a consistent way, advancing quantitative studies of correlated materials.

Superconducting systems may display different types of nonequilibrium states depending on the specific constraints imposed for measurement. We probe current-voltage relations of three-dimensional superconducting films by allowing finite voltages to develop across their length. Our experiments reveal sharp features of negative differential conductance which highlight the validity of the principle of minimum entropy production at the critical current transition. We have observed dissipative states with resistances intermediate between those of superconducting and normal phases at zero applied magnetic field, indicating a phenomenon of phase coexistence under nonequilibrium conditions. The features of steady states reported here are not accessible in conventional transport experiments with current-biasing methods.

The classical Coulomb gas model has served as one of the most versatile frameworks in statistical physics, connecting a vast range of phenomena across many different areas. Nonequilibrium generalisations of this model have so far been studied much more scarcely. With the abundance of contemporary research into active and driven systems, one would naturally expect that such generalisations of systems with long-ranged Coulomb-like interactions will form a fertile playground for interesting developments. Here, we present two examples of novel macroscopic behaviour that arise from nonequilibrium fluctuations in long-range interacting systems, namely (1) unscreened long-ranged correlations in strong electrolytes driven by an external electric field and the associated fluctuation-induced forces in the confined Casimir geometry, and (2) out-of-equilibrium critical behaviour in self-chemotactic models that incorporate the particle polarity in the chemotactic response of the cells. Both of these systems have nonlocal Coulomb-like interactions among their constituent particles, namely, the electrostatic interactions in the case of the driven electrolyte, and the chemotactic forces mediated by fast-diffusing signals in the case of self-chemotactic systems. The results presented here hint to the rich phenomenology of nonequilibrium effects that can arise from strong fluctuations in Coulomb interacting systems, and a rich variety of potential future directions, which are discussed.

Magnetite is an important mineral with many interesting applications related to its magnetic, electrical and thermal properties. Typically studied by electronic structure calculations, these methods are unable to capture the complex ion dynamics at relevant temperatures, time and length scales. We present a hybrid Monte Carlo/Molecular Dynamics (MC/MD) method based on iron oxidation state exchange for accurate atomistic modelling of bulk magnetite, magnetite surfaces and nanoparticles that captures the complex ionic dynamics. By comparing oxidation state patterns with those obtained from density functional theory, we confirmed the accuracy of our approach. Lattice distortions leading to the stabilisation of excess charges and a critical surface thickness at which the oxidation states transition from ordered to disordered were observed. This simple yet efficient approach paves the way for elucidating aspects of oxidation state ordering of inverse spinel structures in general and battery materials in particular.

In a previous study, structure of silica gels prepared in a high magnetic field was investigated. While a direct application of such anisotropic silica gels is for an optical anisotropic medium possessing chemical resistance, we show here their possibility of medium in materials processing. In this direction, for example, silica hydrogels have so far been used as media of crystal growth. In this paper, as opposed to the soft-wet state, dried silica gels have been investigated. We have found that lead (II) nanocrystallites were formed induced by electron irradiation to lead (II)-doped dried silica gels prepared in a high magnetic field such as B = 10 T. Hydrogels made from a sodium metasilicate solution doped with lead (II) acetate were prepared. The dried specimens were irradiated by electrons in a transmission electron microscope environment. Electron diffraction patterns indicated the crystallinity of lead (II) nanocrystallites depending on B. An advantage of this processing technique is that the crystallinity can be controlled through the strength of magnetic field B applied during gel preparation. Specific skills are not required to control the strength of magnetic field.

Two-dimensional (2D) magnetism in atomically thin van der Waals (vdW) monolayers and heterostructures has attracted significant attention due to its promising potential for next-generation spintronic and quantum technologies. A key factor in stabilizing long-range magnetic order in these systems is magnetic anisotropy, which plays a crucial role in overcoming the limitations imposed by the Mermin-Wagner theorem. This review provides a comprehensive theoretical and experimental overview of the importance of magnetic anisotropy in enabling intrinsic 2D magnetism and shaping the electronic, magnetic, and topological properties of 2D vdW materials. We begin by summarizing the fundamental mechanisms that determine magnetic anisotropy, emphasizing the contributions from strong ligand spin-orbit coupling of ligand atoms and unquenched orbital magnetic moments. We then examine a range of material engineering approaches, including alloying, doping, electrostatic gating, strain, and pressure, that have been employed to effectively tune magnetic anisotropy in these materials. Finally, we discuss open challenges and promising future directions in this rapidly advancing field. By presenting a broad perspective on the role of magnetic anisotropy in 2D magnetism, this review aims to stimulate ongoing efforts and new ideas toward the realization of robust, room-temperature applications based on 2D vdW magnetic materials and their heterostructures.

Repeated impacts of a droplet on a vertically forced bath can produce a growing Faraday-wave response under forcing conditions for which the corresponding initially undisturbed bath remains linearly stable. We investigate this mechanism using axisymmetric two-phase direct numerical simulations over a wide range of Reynolds and Weber numbers. The resulting phenomenological regime map identifies quasi-periodic, decaying, faint, and unstable-bath responses. Along the parameter path considered here, the transition to the unstable-bath regime occurs over a narrow range of Weber numbers and varies only weakly with Reynolds number. In the unstable regime, the bath develops a coherent subharmonic response at half the forcing frequency, while disturbances in the decaying regime remain broadband and weaken between successive rebounds. Bath-only simulations show that a finite-amplitude perturbation representative of droplet impact can seed the confined radial mode susceptible to parametric forcing, initiating a growing subharmonic response below the linear instability threshold of the initially flat bath. A reduced capillary-dominated model provides a scaling estimate for the impact-equivalent perturbation amplitude, and bath-only simulations initialized with these perturbations reproduce the bounded-to-growing transition observed in the coupled simulations. Floquet analysis of the finite cylindrical bath identifies the first axisymmetric Neumann mode as having the lowest subharmonic instability threshold. A time-resolved Bessel decomposition independently shows that the growing bath response is dominated by the same radial mode, while the droplet-induced subharmonic response projects predominantly onto this structure. These results identify a finite-amplitude route by which localized droplet impacts can access Faraday-wave dynamics below the linear onset threshold of an initially undisturbed bath.

We investigate the interaction-induced resistivity of ultracold fermions in a three-dimensional optical lattice. In situ observations of transport dynamics enable the determination of real and imaginary resistivity. In the strongly interacting metallic regime, we observe a striking saturation of the current-dissipation rate towards a value that is independent of the interaction strength. This phenomenon is quantitatively captured by a dissipation model that uses a renormalized two-body scattering matrix. We further measure the temperature dependence of resistivity in the strongly interacting limit and discuss the predicted asymptotic high-temperature behavior. Our results provide a clear microscopic understanding of bounded resistivity of low-density metals, thus providing a useful benchmark for studies of strongly correlated atomic and electronic systems.

Here we summarize the physical properties of the newly discovered Fe-chalcogenide superconductors. The Fe-chalcogenide superconductors attract us as the simplest Fe-based superconductors. Furthermore, Fe chalcogenides show a huge pressure effect on their superconducting properties. The origin of the high transition temperature was discussed with both the change in crystal structure and magnetism. The progress on the thin-film and superconducting-wire fabrications are also described.

We propose a self-consistent explanation of Rieger-type periodicities, the Schwabe cycle, and the Suess-de Vries cycle of the solar dynamo in terms of resonances of various wave phenomena with gravitational forces exerted by the orbiting planets. Starting on the high-frequency side, we show that the two-planet spring tides of Venus, Earth and Jupiter are able to excite magneto-Rossby waves which can be linked with typical Rieger-type periods. We argue then that the 11.07-year beat period of those magneto-Rossby waves synchronizes an underlying conventional alpha-Omega-dynamo, by periodically changing either the field storage capacity in the tachocline or some portion of the alpha-effect therein. We also strengthen the argument that the Suess-de Vries cycle appears as an 193-year beat period between the 22.14-year Hale cycle and a spin-orbit coupling effect related with the 19.86-year rosette-like motion of the Sun around the barycenter.

We study linear perturbations of the Maldacena-Milekhin-Popov (MMP) wormhole in the parity sector that pairs axial metric perturbations with polar gauge perturbations. It contains the axial gravitational mode and the electric field along the magnetic field lines. The lowest Landau level (LLL) of the charged fermions responds through its charge. The gauge components a_τ, a_ρ form a two-dimensional gauge field on the worldsheet of each field line, and the fermions respond with the exact Schwinger current. Lifted over the sphere, it gives the electric field the MMP screening mass m_S^2=αq^2, which is not small and survives in the mouth. In the throat the perturbation tilts the worldsheets, and the Casimir stress tensor acquires mixed components. Force balance then requires a current across the field lines, and charge conservation fixes an accompanying polarisation current, the counterpart of the Hall current of the polar sector. These currents close the Bianchi identities at first order in the fermionic backreaction α. The system reduces to three coupled master equations, given in closed form and matched to the fermion-free mouth. Consistency alone does not select the fermionic constitutive relation, but locality, covariance and the index theorem do. At α=0 the throat reduces to Poschl-Teller problems with masses l(l-1) and (l+1)(l+2) at m_S^2=0. At finite m_S^2 one mode is screened, one tends to the mass l^2+l+2, and one neutral charge-density wave stays exactly massless. The O(α) shifts of the massive normal frequencies are real and negative. The two parity sectors are isospectral only without fermions. The neutral channel sees an attractive region in each mouth, and a numerical solution coupled to the gravitational channel in the exact mouth potential finds no bound state. The sector has no growing mode for lge2 at this order.

A stochastic energetics framework is applied to examine how periodically shifting the frequency of a time-dependent oscillating temperature gradient affects heat transport in a nanoscale molecular model. We specifically examine the effects that frequency switching, i.e., instantaneously changing the oscillation frequency of the temperature gradient, has on the shape of the heat transport hysteresis curves generated by a particle connected to two thermal baths, each with a temperature that is oscillating in time. Analytical expressions are derived for the energy fluxes in/out of the system and the baths, with excellent agreement observed between the analytical expressions and the results from nonequilibrium molecular dynamics simulations. We find that the shape of the heat transport hysteresis curves can be significantly altered by shifting the frequency between fast and slow oscillation regimes. We also observe the emergence of features in the hysteresis curves such as pinched loops and complex multi-loop patterns due to the frequency shifting. The presented results have implications in the design of thermal neuromorphic devices such as thermal memristors and thermal memcapacitors.

The ionosphere electromagnetic activity is a major factor of the quality of satellite telecommunications, Global Navigation Satellite Systems (GNSS) and other vital space applications. Being able to forecast globally the Total Electron Content (TEC) would enable a better anticipation of potential performance degradations. A few studies have proposed models able to predict the TEC locally, but not worldwide for most of them. Thanks to a large record of past TEC maps publicly available, we propose a method based on Deep Neural Networks (DNN) to forecast a sequence of global TEC maps consecutive to an input sequence of TEC maps, without introducing any prior knowledge other than Earth rotation periodicity. By combining several state-of-the-art architectures, the proposed approach is competitive with previous works on TEC forecasting while predicting the TEC globally.

Spintronics is expected as the next-generation technology based on the novel notch of spin degree of freedom of electrons. Half metals, a class of materials which behave as a metal in one spin direction and an insulator in the opposite spin direction, are ideal for spintronic applications. Half metallic antiferromagnets as a subclass of half metals are characterized further by totally compensated spin moments in a unit cell, and have the advantage of being able to generate fully spin-polarized current while exhibiting zero macroscopic magnetization. Considerable efforts have been devoted to the search for this novel material, from which we may get useful hints for prospective material exploration.

Chiral magnons, the quanta of handed spin waves, transport spin angular momentum without energy loss due to Joule heating. The recently discovered altermagnets were proposed to host chiral magnons arising from a non-relativistic exchange mechanism, similar to that in ferromagnets but without net magnetization, offering a stray-field-free platform for efficient magnon spin-current manipulation. In this work, we directly observed chiral magnons in the altermagnetic prototype MnTe using polarized inelastic neutron scattering. Furthermore, the magnon chirality was found to be reversibly switched by magnetic-field control, establishing a robust foundation for functional altermagnetic magnonics.

An experimental demonstration of directivities exceeding the fundamental Kildal limit, a phenomenon called superdirectivity, is provided for spherical high-index dielectric antennas with an electric dipole excitation. A directivity factor of about 10 with a total efficiency of more than 80\% for an antenna having a size of a third of the wavelength was measured. High directivities are shown to be associated with constructive interference of particular electric and magnetic modes of an open spherical resonator. Both analytic solution for a point dipole and a full-wave rigorous simulation for a realistic dipole antenna were employed for optimization and analysis, yielding an excellent agreement between experimentally measured and numerically predicted directivities. The use of high-index low-loss ceramics can significantly reduce the physical size of such antennas while maintaining their overall high radiation efficiency. Such antennas can be attractive for various high-frequency applications, such as antennas for the Internet of things, smart city systems, 5G network systems, and others. The demonstrated concept can be scaled in frequency.

This paper concerns the derivation of radiative transfer equations for acoustic waves propagating in a randomly fluctuating slab (between two parallel planes) in the weak-scattering regime, and the study of boundary effects through an asymptotic analysis of the Wigner transform of the wave solution. These radiative transfer equations allow to model the transport of wave energy density, taking into account the scattering by random heterogeneities. The approach builds on the method of images, where the slab is extended to a full-space, with a periodic map of mechanical properties and a series of sources located along a periodic pattern. Two types of boundary effects, both on the (small) scale of the wavelength, are observed: one at the boundaries of the slab, and one inside the domain. The former impact the entire energy density (coherent as well as incoherent) and is also observed in half-spaces. The latter, more specific to slabs, corresponds to the constructive interference of waves that have reflected at least twice on the boundaries of the slab and only impacts the coherent part of the energy density.

We show that a simple gravitational theory can provide a holographically dual description of a superconductor. There is a critical temperature, below which a charged condensate forms via a second order phase transition and the (DC) conductivity becomes infinite. The frequency dependent conductivity develops a gap determined by the condensate. We find evidence that the condensate consists of pairs of quasiparticles.

Ferrofluids show unusual hydrodynamic effects due to the magnetic nature of their constituents. For increasing magnetization a classical ferrofluid undergoes a Rosensweig instability and creates self-organized ordered surface structures or droplet crystals. A Bose-Einstein condensate with strong dipolar interactions is a quantum ferrofluid that also shows superfluidity. The field of dipolar quantum gases is motivated by the search for new phases that break continuous symmetries. The simultaneous breaking of continuous symmetries like the phase invariance for the superfluid state and the translational symmetry for a crystal provides the basis of novel states of matter. However, interaction-induced crystallization in a superfluid has not been observed. Here we use in situ imaging to directly observe the spontaneous transition from an unstructured superfluid to an ordered arrangement of droplets in an atomic dysprosium Bose-Einstein condensate. By utilizing a Feshbach resonance to control the interparticle interactions, we induce a finite-wavelength instability and observe discrete droplets in a triangular structure, growing with increasing atom number. We find that these states are surprisingly long-lived and measure a hysteretic behaviour, which is typical for a crystallization process and in close analogy to the Rosensweig instability. Our system can show both superfluidity and, as shown here, spontaneous translational symmetry breaking. The presented observations do not probe superfluidity in the structured states, but if the droplets establish a common phase via weak links, this system is a very good candidate for a supersolid ground state.

We have investigated the effects of strain on two-dimensional square lattices and examined the methods for inducing pseudo-magnetic fields. In both the columnar and staggered pi-flux square lattices, we have found that strain only modulates Fermi velocities rather than inducing pseudo-magnetic fields. However, spatially non-uniform on-site potentials (anisotropic hoppings) can create pseudo-magnetic fields in columnar (staggered) pi-flux square lattices. On the other hand, we demonstrate that strain does induce pseudo-magnetic fields in staggered zero-flux square lattices. By breaking a quarter of the bonds, we clarify that a staggered zero-flux square lattice is topologically equivalent to a honeycomb lattice and displays pseudo-vector potentials and pseudo-Landau levels at the Dirac points.

The intricate relationship between electrons and the crystal lattice is a linchpin in condensed matter, traditionally described by the Fr\"ohlich model encompassing the lowest-order lattice-electron coupling. Recently developed quantum acoustics, emphasizing the wave nature of lattice vibrations, has enabled the exploration of previously uncharted territories of electron-lattice interaction not accessible with conventional tools such as perturbation theory. In this context, our agenda here is two-fold. First, we showcase the application of machine learning methods to categorize various interaction regimes within the subtle interplay of electrons and the dynamical lattice landscape. Second, we shed light on a nebulous region of electron dynamics identified by the machine learning approach and then attribute it to transient localization, where strong lattice vibrations result in a momentary Anderson prison for electronic wavepackets, which are later released by the evolution of the lattice. Overall, our research illuminates the spectrum of dynamics within the Fr\"ohlich model, such as transient localization, which has been suggested as a pivotal factor contributing to the mysteries surrounding strange metals. Furthermore, this paves the way for utilizing time-dependent perspectives in machine learning techniques for designing materials with tailored electron-lattice properties.

The simulation of large-scale systems with complex electron interactions remains one of the greatest challenges for the atomistic modeling of materials. Although classical force fields often fail to describe the coupling between electronic states and ionic rearrangements, the more accurate ab-initio molecular dynamics suffers from computational complexity that prevents long-time and large-scale simulations, which are essential to study many technologically relevant phenomena, such as reactions, ion migrations, phase transformations, and degradation. In this work, we present the Crystal Hamiltonian Graph neural Network (CHGNet) as a novel machine-learning interatomic potential (MLIP), using a graph-neural-network-based force field to model a universal potential energy surface. CHGNet is pretrained on the energies, forces, stresses, and magnetic moments from the Materials Project Trajectory Dataset, which consists of over 10 years of density functional theory static and relaxation trajectories of sim 1.5 million inorganic structures. The explicit inclusion of magnetic moments enables CHGNet to learn and accurately represent the orbital occupancy of electrons, enhancing its capability to describe both atomic and electronic degrees of freedom. We demonstrate several applications of CHGNet in solid-state materials, including charge-informed molecular dynamics in Li_xMnO_2, the finite temperature phase diagram for Li_xFePO_4 and Li diffusion in garnet conductors. We critically analyze the significance of including charge information for capturing appropriate chemistry, and we provide new insights into ionic systems with additional electronic degrees of freedom that can not be observed by previous MLIPs.

At high energies, the dynamics of a plasma with charged fermions can be described in terms of chiral magnetohydrodynamics. Using direct numerical simulations, we demonstrate that chiral magnetic waves (CMWs) can produce a chiral asymmetry μ_5 = μ_L - μ_R from a spatially fluctuating (inhomogeneous) chemical potential μ= μ_L + μ_R, where μ_L and μ_R are the chemical potentials of left- and right-handed electrically charged fermions, respectively. If the frequency of the CMW is less than or comparable to the characteristic growth rate of the chiral dynamo instability, the magnetic field can be amplified on small spatial scales. The growth rate of this small-scale chiral dynamo instability is determined by the spatial maximum value of μ_5 fluctuations. Therefore, the magnetic field amplification occurs during periods when μ_5 reaches temporal maxima during the CMW. If the small-scale chiral dynamo instability leads to a magnetic field strength that exceeds a critical value, which depends on the resistivity and the initial value of μ, magnetically dominated turbulence is produced. Turbulence gives rise to a large-scale dynamo instability, which we find to be caused by the magnetic alpha effect. Our results have consequences for the dynamics of certain high-energy plasmas, such as the early Universe.

We demonstrate an all solid state semiconductor device, based on epitaxial single crystalline metal halide perovskites, enabling reversible control of a perovskite photoluminescence with a gate voltage. Fundamentally distinct from electroluminescent diodes, such a photoluminescence field effect transistor uses the gate electric field to electrostatically modulate the interfacial density of mobile charges, thereby affecting the radiative and nonradiative recombination channels of photocarriers. Varying the gate voltage in such transistors efficiently changes the rate of nonradiative interfacial recombination and modulates the photoluminescence intensity by 65 to 98 percent (depending on temperature). At favorable gating, nearly complete elimination of non-radiative losses can be achieved. This functionality, coupled with the strong visible-range absorption and emission, possible due to the high absorption coefficient, as well as controllable thickness and macroscopically homogeneous morphology of epitaxial perovskite films, leads to high external photoluminescence quantum efficiencies realized in large-area, thin-film devices. Such high-efficiency, scalable, electrostatically tunable optoelectronic switches broaden the potential applications of metal-halide perovskites in photonics and optoelectronics.

We investigate inflationary magnetogenesis with massive vector fields, including charged scalar particle production via the Schwinger effect and its backreaction on the background electric energy density. Initially neglecting the Schwinger effect, we quantize the vector field and solve the equations of motion for transverse and longitudinal modes, computing the energy momentum tensor. We then incorporate the backreaction of the electric energy density and show that the longitudinal energy density is subleading compared to the electric background. Since the electric energy density dominates the magnetic contribution, we can treat the former separately from the perturbative contributions. We adopt this approach when studying particle production via the Schwinger effect, assuming that its backreaction acts only on the background electric energy density. The latter is computed using a classical background electromagnetic field minimally coupled to a quantum complex scalar field. The magnetic and longitudinal components are instead described through quantum fields. In this framework, the Schwinger production affects only the electric energy density, as long as it remains dominant compared to the other components. As a consistency check, we verify that for a null coupling constant we recover the same electric energy density as obtained within the fully quantum electromagnetic description. Finally, we show that for non-null coupling constants Schwinger particle production drastically reduces the electric energy density during the final stages of inflation.

We study photon conversion into light particles, such as dilatons, axions, and gravitons, induced by background magnetic fields, and formulate the resulting evolution in terms of the Stokes parameters. We show that photon conversion reduces to an effective non-unitary evolution of the photon sector. In the perturbative regime, the Hermitian and anti-Hermitian parts of the effective photon Hamiltonian are related through Kramers--Kronig relations, revealing that the changes in the Stokes parameters are not independent. We apply this general framework to photon evolution in Gaussian stochastic magnetic fields with possible helicity, and derive the ensemble-averaged evolution of the Stokes parameters. We find that two nonzero contributions arise even in the absence of magnetic helicity, which respectively correspond to the overall attenuation of all the Stokes parameters and to an irrelevant overall phase. We also find that magnetic helicity gives rise to two additional contributions, one of which changes the circular polarization while the other induces a rotation of linear polarization. These contributions form two Kramers--Kronig pairs. In particular, photon conversion induced by magnetic helicity is accompanied by both circular-polarization and birefringent responses. The same structure appears in dilaton-photon, axion-photon, and graviton-photon systems, revealing universality of photon conversion in magnetic fields.

Hexagonal oxide perovskites, in contrast to the more familiar perovskites, allow for face-sharing of metal-oxygen octahedra or trigonal prisms within their structural frameworks. This results in dimers, trimers, tetramers, or longer fragments of chains of face-sharing octahedra in the crystal structures, and consequently in much shorter metal-metal distances and lower metal-oxygen-metal bond angles than are seen in the more familiar perovskites. The presence of the face-sharing octahedra can have a dramatic impact on magnetic properties of these compounds, and dimer-based materials, in particular, have been the subjects of many quantum-materials-directed studies in materials physics. Hexagonal oxide perovskites are of contemporary interest due to their potential for geometrical frustration of the ordering of magnetic moments or orbital occupancies at low temperatures, which is especially relevant to their significance as quantum materials. As such, several hexagonal oxide perovskites have been identified as potential candidates for hosting the quantum spin liquid state at low temperatures. In our view, hexagonal oxide perovskites are fertile ground for finding new quantum materials. This review briefly describes the solid state chemistry of many of these materials.

Topological aspects of the geometry of DNA and similar chiral molecules have received a lot of attention, while the topology of their electronic structure is less explored. Previous experiments have revealed that DNA can efficiently filter spin-polarized electrons between metal contacts, a process called chiral-induced spin-selectivity (CISS). However, the underlying correlation between chiral structure and electronic spin remains elusive. In this work, we reveal an orbital texture in the band structure, a topological characteristic induced by the chirality. We find that this orbital texture enables the chiral molecule to polarize the quantum orbital. This orbital polarization effect (OPE) induces spin polarization assisted by the spin-orbit interaction from a metal contact and leads to magnetorestistance and chiral separation. The orbital angular momentum of photoelectrons also plays an essential role in related photoemission experiments. Beyond CISS, we predict that OPE can induce spin-selective phenomena even in achiral but inversion-breaking materials.