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2005-11-19
Transport, thermal and magnetic properties of RuSr_2(Gd_{1.5}Ce_{0.5})Cu_2O_{10-δ}, a magnetic superconductor
Resistivity, thermoelectric power, heat capacity and magnetization for samples of RuSr_2(Gd_{1.5}Ce_{0.5})Cu_{2}O_{10-\delta} were investigated in the temperature range 1.8-300 K with a magnetic field up to 8 T. The resistive transitions to the superconducting state are found to be determined by the inhomogeneous (granular) structure, characterized by the intragranular, T_{c0}, and intergranular, T_{cg}, transition temperatures. Heat capacity, C(T), shows a jump at the superconducting transition temperature T_{c0}\approx 37.5 K. A Schottky-like anomaly is found in C(T) below 20 K. This low temperature anomaly can be attributed to splitting of the ground term $^{8}S_{7/2}$ of paramagnetic Gd^{3+} ions by internal and external magnetic fields.
0511489v1
2007-03-28
Comparison between experiment and calculated band structures for DyN and SmN
We investigate the electronic band structure of two of the rare-earth nitrides, DyN and SmN. Resistivity measurements imply that both materials have a semiconducting ground state, and both show resistivity anomalies coinciding with the magnetic transition, despite the different magnetic states in DyN and SmN. X-ray absorption and emission measurements are in excellent agreement with LSDA+U calculations, although for SmN the calculations predict a zero band gap.
0703740v3
2007-04-24
Impedance spectroscopy of epitaxial multiferroic thin films
Temperature dependent impedance spectroscopy enables the many contributions to the dielectric and resistive properties of condensed matter to be deconvoluted and characterized separately. We have achieved this for multiferroic epitaxial thin films of BiFeO3 (BFO) and BiMnO3 (BMO), key examples of materials with strong magneto-electric coupling. We demonstrate that the true film capacitance of the epitaxial layers is similar to that of the electrode interface, making analysis of capacitance as a function of film thickness necessary to achieve deconvolution. We modeled non-Debye impedance response using Gaussian distributions of relaxation times and reveal that conventional resistivity measurements on multiferroic layers may be dominated by interface effects. Thermally activated charge transport models yielded activation energies of 0.60 eV +- 0.05 eV (BFO) and 0.25 eV +- 0.03 eV (BMO), which is consistent with conduction dominated by oxygen vacancies (BFO) and electron hopping (BMO). The intrinsic film dielectric constants were determined to be 320 +- 75 (BFO) and 450 +- 100 (BMO).
0704.3262v1
2007-08-09
Carbon nanotube array vias for interconnect applications
The material and electrical properties of the CNT single vias and array vias grown by microwave plasma-enhanced chemical vapor deposition were investigated. The diameters of multiwall carbon nanotubes (MWNTs) grown on the bottom electrode of Ta decrease with increasing pretreatment power and substrate temperature while the effects of the growth power and methane flow ratio are insignificant The decrease of CNT diameters leads to the decrease of the CNT via diode devices. The increase of growth power enhances the CNT graphitization degree and thue the conductivity of CNT via diode devices. In the same via region, the MWNT diode resistances of the array vias are lower than those of the single vias. The MWNT diode resistances on the bottom electrode of titanium are lower than those on the bottom electrode of tantalum. It may be attributed to the smaller tube diameters on the bottom electrode of Ti and the work function difference between Ta and Ti films with respect to the work function of CNTs.
0708.1298v1
2007-08-14
Suspension of Nanoparticles in SU-8 and Characterization of Nanocomposite Properties
Gold nanospheres, single wall carbon nanotubes (SWNT), and diamonoids were phyically incorporated into the negative photoresist SU-8. the mixtures were spin cast onto silicon or aluminium coated silicon wafers. ASTM standard D638 tensile specimens were lithographically patterned in the materials and then released from the substrate using Microchem'Omnicoat or an anodic metal dissolution process. the residual stresses, elastic moduli, and viscosity of the SU-8. Resistivity measurements of SU-8/SWNT nanocomposites were also investigates. We found the effective modulus and viscosity of the SU-8 test specimens decreases with the addition of diamantane and SWNTs. Additionally, the SU-8/SWNT nanocomposites showed changes in resistivity with increased strain, suggesting a gauge factor for the 1 wt% SU-8/SWNT nanocomposite of approximately 2-4.
0708.1822v1
2007-12-07
Field Tuned Superconductor to Insulator Transitions in an Amorphous Film with an Imposed Multiply Connected Geometry
We have observed multiple magnetic field driven superconductor to insulator transitions (SIT) in amorphous Bi films perforated with a nano-honeycomb (NHC) array of holes. The period of the magneto-resistance, H=H_M=h/2eS where S is the area of a unit cell of holes, indicates the field driven transitions are boson dominated. The field-dependent resistance follows R(T)=R_0(H)exp(T_0(H)/T) on both sides of the transition so that the evolution between these states is controlled by the vanishing of T_0 to0. We compare our results to the thickness driven transition in NHC films and the field driven transitions in unpatterned Bi films, other materials, and Josephson junction arrays. Our results suggest a structural source for similar behavior found in some materials and that despite the clear bosonic nature of the SITs, quasiparticle degrees of freedom likely also play an important part in the evolution of the SIT.
0712.1076v1
2008-07-02
Nano Imprint Lithography on Silica Sol-gels: a simple route to sequential patterning
Since the pioneering work of S.Y. Chou et al.[1] Nano Imprint Lithography (NIL) has emerged as a promising technique for surface patterning, opening for numerous applications ranging from nanophotonics[2] to microfluidics[3]. NIL basically consists in the stamping of deformable surfaces or films. Preferred materials are thermoplastics[4] and UV curable resists[5]. So far, most papers report on single imprinting methods for which the same surface is imprinted only once. In the present paper, we report the imprinting of square silica structures from simple line gratings and demonstrate how the specific thermo-rheological behavior of ICSG resists can be harnessed to form complex structures by sequential imprinting at low pressures.
0807.0378v1
2009-01-09
Stability of a Charged Particle Beam in a Resistive Plasma Channel
A self-focusing of a coasting relativistic beam in a plasma channel that is confined by an external magnetic field is studied as a means of reconditioning the beam emerging from a beam injector [a radio frequency quadrupole (RFQ)] for a linac. A detailed study of the beam stability in the self-focused beam has been carried out. In order to explain beam filaments and the resistive hose instability in a unified way, we treat all the azimuthal modes in the derivation of the dispersion relation in a finite plasma channel that exhibit many unstable modes, which are classified by Weinberg's scheme [Steven Weinberg, J. Math. 8, 614 (1967)].
0901.1167v2
2009-07-21
Anomalous transport properties of the halfmetallic ferromagnets Co2TiSi, Co2TiGe, and Co2TiSn
In this work the theoretical and experimental investigations of Co2TiZ (Z = Si, Ge, or Sn) compounds are reported. Half-metallic ferromagnetism is predicted for all three compounds with only two bands crossing the Fermi energy in the majority channel. The magnetic moments fulfill the Slater-Pauling rule and the Curie temperatures are well above room temperature. All compounds show a metallic like resistivity for low temperatures up to their Curie temperature, above the resistivity changes to semiconducting like behavior. A large negative magnetoresistance of 55% is observed for Co2TiSn at room temperature in an applied magnetic field of 4T which is comparable to the large negative magnetoresistances of the manganites. The Seebeck coefficients are negative for all three compounds and reach their maximum values at their respective Curie temperatures and stay almost constant up to 950 K. The highest value achieved is -52muV/K m for Co2TiSn which is large for a metal. The combination of half-metallicity and the constant large Seebeck coefficient over a wide temperature range makes these compounds interesting materials for thermoelectric applications and further spincaloric investigations.
0907.3562v1
2009-08-27
A low field technique for measuring magnetic and magneto-resistance anisotropy coefficients applied to (Ga,Mn)As
We demonstrate a simple, low cost, magneto-transport method for rapidly characterizing the magnetic anisotropy and anisotropic magneto-resistance (AMR) of ferromagnetic devices with uniaxial magnetic anisotropy. This transport technique is the analogue of magnetic susceptibility measurements of bulk material but is applicable to very small samples with low total moment. The technique is used to characterize devices fabricated from the dilute magnetic semiconductor (Ga,Mn)As. The technique allows us to probe the behavior of the parameters close to the Curie temperature, in the limit of the applied magnetic field tending to zero. This avoids the complications arising from the presence of paramagnetism.
0908.3960v1
2010-01-20
Robust charge and magnetic order under electric field and current in the multiferroic LuFe(2)O(4)
We performed elastic neutron scattering measurements on the charge- and magnetically-ordered multiferroic material LuFe(2)O(4). An external electric field along the [001] direction with strength up to 20 kV/cm applied at low temperature (~100 K) does not affect either the charge or magnetic structure. At higher temperatures (~360 K), before the transition to three-dimensional charge-ordered state, the resistivity of the sample is low, and an electric current was applied instead. A reduction of the charge and magnetic peak intensities occurs when the sample is cooled under a constant electric current. However, after calibrating the real sample temperature using its own resistance-temperature curve, we show that the actual sample temperature is higher than the thermometer readings, and the "intensity reduction" is entirely due to internal sample heating by the applied current. Our results suggest that the charge and magnetic orders in LuFe(2)O(4) are unaffected by the application of external electric field/current, and previously observed electric field/current effects can be naturally explained by internal sample heating.
1001.3611v2
2010-10-07
Compensation-dependence of magnetic and electrical properties in Ga1-xMnxP
We demonstrate the control of the hole concentration in Ga1-xMnxP over a wide range by introducing compensating vacancies. The resulting evolution of the Curie temperature from 51 K to 7.5 K is remarkably similar to that observed in Ga1-xMnxAs despite the dramatically different character of hole transport between the two material systems. The highly localized nature of holes in Ga1-xMnxP is reflected in the accompanying increase in resistivity by many orders of magnitude. Based on variable-temperature resistivity data we present a general picture for hole conduction in which variable-range hopping is the dominant transport mechanism in the presence of compensation.
1010.1368v2
2011-02-04
Low-Frequency Current Fluctuations in Graphene-like Exfoliated Thin-Films of Topological Insulators
We report on the low-frequency current fluctuations and electronic noise in thin-films made of bismuth selenide topological insulators. The films were prepared via the graphene-like mechanical exfoliation and used as the current conducting channels in the four- and two-contact devices. Analysis of the resistance dependence on the film thickness indicates that the surface contribution to conductance is dominant in our samples. It was established that the current fluctuations have the noise spectrum close to the pure 1/f in the frequency range from 1 to 10 kHz (f is the frequency). The relative noise amplitude S/I^2 for the examined films was increasing from ~5x10^-8 to 5x10^-6 (1/Hz) as the resistance of the channels varied from ~10^3 to 10^5 Ohms. The obtained noise data is important for understanding electron transport through the surface and volume of topological insulators, and proposed applications of this class of materials.
1102.0961v1
2011-05-04
Sondheimer Oscillation as a Fingerprint of Surface Dirac Fermions
Topological states of matter challenge the paradigm of symmetry breaking, characterized by gapless boundary modes and protected by the topological property of the ground state. Recently, angle-resolved photoemission spectroscopy (ARPES) has revealed that semiconductors of Bi$_{2}$Se$_{3}$ and Bi$_{2}$Te$_{3}$ belong to such a class of materials. Here, we present undisputable evidence for the existence of gapless surface Dirac fermions from transport in Bi$_{2}$Te$_{3}$. We observe Sondheimer oscillation in magnetoresistance (MR). This oscillation originates from the quantization of motion due to the confinement of electrons within the surface layer. Based on Sondheimer's transport theory, we determine the thickness of the surface state from the oscillation data. In addition, we uncover the topological nature of the surface state, fitting consistently both the non-oscillatory part of MR and the Hall resistance. The side-jump contribution turns out to dominate around 1 T in Hall resistance while the Berry-curvature effect dominates in 3 T $\sim$ 4 T.
1105.0731v1
2011-07-05
Evidence for filamentary superconductivity nucleated at antiphase domain walls in antiferromagnetic CaFe$_2$As$_2$
Resistivity, magnetization and microscopic $^{75}$As nuclear magnetic resonance (NMR) measurements in the antiferromagnetically ordered state of the iron-based superconductor parent material CaFe$_2$As$_2$ exhibit anomalous features that are consistent with the collective freezing of domain walls. Below $T^*\approx 10$ K, the resistivity exhibits a peak and downturn, the bulk magnetization exhibits a sharp increase, and $^{75}$As NMR measurements reveal the presence of slow fluctuations of the hyperfine field. These features in both the charge and spin response are strongly field dependent, are fully suppressed by $H^*\approx 15$ T, and suggest the presence of filamentary superconductivity nucleated at the antiphase domain walls in this material.
1107.0904v2
2011-08-22
Ferromagnetic Quantum Criticality in the Quasi-One-Dimensional Heavy Fermion Metal YbNi4P2
We present a new Kondo-lattice system, YbNi4P2, which is a clean heavy-fermion metal with a severely reduced ferromagnetic ordering temperature at T_C=0.17K, evidenced by distinct anomalies in susceptibility, specific-heat, and resistivity measurements. The ferromagnetic nature of the transition, with only a small ordered moment of ~0.05mu_B, is established by a diverging susceptibility at T_C with huge absolute values in the ferromagnetically ordered state, severely reduced by small magnetic fields. Furthermore, YbNi4P2 is a stoichiometric system with a quasi-one-dimensional crystal and electronic structure and strong correlation effects which dominate the low temperature properties. This is reflected by a stronger-than-logarithmically diverging Sommerfeld coefficient and a linear-in-T resistivity above T_C which cannot be explained by any current theoretical predictions. These exciting characteristics are unique among all correlated electron systems and make this an interesting material for further in-depth investigations.
1108.4274v1
2012-10-18
Observation of a Large Photo-response in a Single Nanowire (Diameter ~30 nm) of Charge Transfer Complex Cu:TCNQ
We report for the first time large photoresponse in a single NW of the charge transfer complex Cu:TCNQ. We fabricate a metal-semiconductor-metal device with a single NW and focus ion beam deposited Pt. We observe large photocurrent even at zero bias. The spectral dependence of the photoresponse follows the main absorption at ~ 405 nm which has the primarily responsible for photogenerated carriers. We have quantitatively analyzed the bias dependent photocurrent by a model of two back to back Schottky diodes connected by a series resistance. The observation shows that the large photoresponse of the device primarily occurs due to the reduction of the barrier at the contact regions due to illumination along with the photoconductive contribution. There is also a bias driven reduction of the nanowire resistance that is a unique feature for the material.
1210.5207v1
2013-01-16
Huge field-effect surface charge injection and conductance modulation in metallic thin films by electrochemical gating
The field-effect technique, popular thanks to its application in common field-effect transistors, is here applied to metallic thin films by using as a dielectric a novel polymer electrolyte solution. The maximum injected surface charge, determined by a suitable modification of a classic method of electrochemistry called double-step chronocoulometry, reached some units in 10^15 charges/cm^2. At room temperature, relative variations of resistance up to 8%, 1.9% and 1.6% were observed in the case of gold, silver and copper, respectively and, if the films are thick enough (> 25 nm), results can be nicely explained within a free-electron model with parallel resistive channels. The huge charge injections achieved make this particular field-effect technique very promising for a vast variety of materials such as unconventional superconductors, graphene and 2D-like materials.
1301.3769v1
2013-02-05
Scaling of Non-Saturating MR and quantum oscillations in pristine and ion-implanted HOPG
A wide variety of resistive and field dependent behaviors have been previously observed in both doped and non-doped Highly Oriented Pyrolytic Graphite (HOPG). We find HOPG samples to vary significantly in their temperature dependent resistances, even between portions taken from the same sample, yet they exhibit consistent non-saturating magnetoresistance (MR). The scaling behavior of the MR is shown to be characteristic of a model based on the Hall effect in granular materials. In addition to the large, field-linear MR, all samples exhibit Shubnikov-de Haas (SdH) oscillations. Additional samples were doped via ion-implantation by boron and phosphorous, but show no signs of superconductivity nor any systematic change in their magnetoresistive behavior. Analysis of the SdH data gives a 2D carrier density in agreement with previous results, and a large mean-free path relative to crystallite size, even in samples with thin ion-implanted surface layers.
1302.1229v1
2013-02-07
Thermoelectromotive force of hafnium at plastic deformation in regime of creep at temperature of 300 K
The thermoelectromotive force and electrical resistivity of the polycrystalline hafnium (Hf) with the grain size of 10 {\mu}m during the process of plastic deformation in the regime of creep at the temperature of 300 K are precisely measured. It is shown that the thermoelectromotive force depends on the deformation mechanism nature, because of the changing magnitude of the electrons scattering on the different structural defects in the hafnium crystal lattice at the deformation process. The main research conclusion is that the method of thermoelectromotive force measurements is more informative, comparing to the method of electric resistivity measurements in the process of accurate characterization of the hafnium.
1302.1784v1
2013-03-11
Nanobatteries in redox-based resistive switches require extension of memristor theory
Redox-based nanoionic resistive memory cells (ReRAMs) are one of the most promising emerging nano-devices for future information technology with applications for memory, logic and neuromorphic computing. Recently, the serendipitous discovery of the link between ReRAMs and memristors and memristive devices has further intensified the research in this field. Here we show on both a theoretical and an experimental level that nanoionic-type memristive elements are inherently controlled by non-equilibrium states resulting in a nanobattery. As a result the memristor theory must be extended to fit the observed non zerocrossing I-V characteristics. The initial electromotive force of the nanobattery depends on the chemistry and the transport properties of the materials system but can also be introduced during ReRAM cell operations. The emf has a strong impact on the dynamic behaviour of nanoscale memories, and thus, its control is one of the key factors for future device development and accurate modelling.
1303.2589v1
2013-07-02
Non-volatile ferroelastic switching of the Verwey transition and resistivity of epitaxial Fe3O4/PMN-PT (011)
A central goal of electronics based on correlated materials or 'Mottronics' is the ability to switch between distinct collective states with a control voltage. Small changes in structure and charge density near a transition can tip the balance between competing phases, leading to dramatic changes in electronic and magnetic properties. In this work, we demonstrate that an electric field induced two-step ferroelastic switching pathway in (011) oriented 0.71Pb(Mg1/3Nb2/3)O3-0.29PbTiO3 (PMN-PT) substrates can be used to tune the Verwey metal-insulator transition in epitaxial Fe3O4 films in a stable and reversible manner. We also observe robust non-volatile resistance switching in Fe3O4 up to room temperature, driven by ferroelastic strain. These results provides a framework for realizing non-volatile and reversible tuning of order parameters coupled to lattice-strain in epitaxial oxide heterostructures over a broad range of temperatures, with potential device applications.
1307.0838v1
2014-06-01
Effect of carrier concentration on magnetism and magnetic order in the pyrochlore iridates
We present resistivity, magnetization, and zero field muon spin relaxation ($\mu$SR) data for the pyrochlore iridate materials Nd$_{2-x}$Ca$_{x}$Ir$_{2}$O$_{7}$ ($x = 0, 0.06$, and $0.10$) and Sm$_2$Ir$_2$O$_7$. While Nd$_{2}$Ir$_{2}$O$_{7}$ (Nd227) is weakly conducting, Sm$_{2}$Ir$_{2}$O$_{7}$ (Sm227) has slowly diverging resistivity at low temperature. Nd227 and Sm227 exhibit magnetic anomalies at $T_{M} = 105 K$ and $137 K$, respectively. However, zero-field $\mu$SR measurements show that long-range magnetic order of the Ir$^{4+}$ sublattice sets in at much lower temperatures ($T_{LRO} \sim 8 K$ for Nd227 and $70 K$ for Sm227); both materials show heavily damped muon precession with a characteristic frequency near 9 MHz. The magnetic anomaly at $T_{M}$ in Nd227 is not significantly affected by the introduction of hole carriers by Ca-substitution in the conducting Nd$_{2-x}$Ca$_{x}$Ir$_{2}$O$_{7}$ samples, but the muon precession is fully suppressed for both.
1406.0194v1
2014-10-07
Thickness Scaling Effect on Interfacial Barrier and Electrical Contact to Two-Dimensional MoS2 Layers
Understanding the interfacial electrical properties between metallic electrodes and low dimensional semiconductors is essential for both fundamental science and practical applications. Here we report the observation of thickness reduction induced crossover of electrical contact at Au/MoS2 interfaces. For MoS2 thicker than 5 layers, the contact resistivity slightly decreases with reducing MoS2 thickness. By contrast, the contact resistivity sharply increases with reducing MoS2 thickness below 5 layers, mainly governed by the quantum confinement effect. It is found that the interfacial potential barrier can be finely tailored from 0.3 to 0.6 eV by merely varying MoS2 thickness. A full evolution diagram of energy level alignment is also drawn to elucidate the thickness scaling effect. The finding of tailoring interfacial properties with channel thickness represents a useful approach controlling the metal/semiconductor interfaces which may result in conceptually innovative functionalities.
1410.1943v2
2015-03-04
Observation of the chiral anomaly induced negative magneto-resistance in 3D Weyl semi-metal TaAs
Weyl semi-metal is the three dimensional analog of graphene. According to the quantum field theory, the appearance of Weyl points near the Fermi level will cause novel transport phenomena related to chiral anomaly. In the present paper, we report the first experimental evidence for the long-anticipated negative magneto-resistance generated by the chiral anomaly in a newly predicted time-reversal invariant Weyl semi-metal material TaAs. Clear Shubnikov de Haas oscillations (SdH) have been detected starting from very weak magnetic field. Analysis of the SdH peaks gives the Berry phase accumulated along the cyclotron orbits to be {\pi}, indicating the existence of Weyl points.
1503.01304v1
2015-03-12
Shubnikov-de Haas oscillations, weak antilocalization effect and large linear magnetoresistance in the putative topological superconductor LuPdBi
We present electronic transport and magnetic properties of single crystals of semimetallic half-Heusler phase LuPdBi, having theoretically predicted band inversion requisite for nontrivial topological properties. The compound exhibits superconductivity below a critical temperature $T_{\rm c}=1.8\,$K, with a zero-temperature upper critical field $B_{\rm c2}\approx2.3\,$T. Although superconducting state is clearly reflected in the electrical resistivity and magnetic susceptibility data, no corresponding anomaly can be seen in the specific heat. Temperature dependence of the electrical resistivity suggests existence of two parallel conduction channels: metallic and semiconducting, with the latter making negligible contribution at low temperatures. The magnetoresistance is huge and clearly shows a weak antilocalization effect in small magnetic fields. Above about 1.5 T, the magnetoresistance becomes linear and does not saturate in fields up to 9 T. The linear magnetoresistance is observed up to room temperature. Below 10 K, it is accompanied by Shubnikov-de Haas oscillations. Their analysis reveals charge carriers with effective mass of $0.06\,m_e$ and a Berry phase very close to $\pi$, expected for Dirac-fermion surface states, thus corroborating topological nature of the material.
1503.03697v1
2015-11-17
Microstructure, mechanical properties and corrosion of friction stir welded 6061 Aluminum Alloy
The microstructure, mechanical properties, and corrosion behavior of friction stir welded (FSW) AA6061 aluminum alloys were investigated. Dynamic recrystallized structures were observed and grain sizes of nugget zone (NZ), thermomechanically-affected zone (TMAZ), heat-affected zone (HAZ), and base material (BM) were different. Hardness test indicated that the minimum and maximum hardness values wereobtained in the HAZ and BM, respectively. Tensile results showed that fracture occurred in the relatively weak regions in between TMAZ and HAZ. Polarization tests illustrated that the FSW process improved the corrosion resistance of AA6061-AA6061 and the HAZ had better corrosion resistance than other regions. Raman characterizations revealed that aluminum hydroxide was the main corrosion product formed on Al after immersion experiments. Intergranular attack was observed in the NZ and downside by scanning electron microscopy.
1511.05507v1
2015-11-20
Transmission conditions for thin curvilinear close to circular heat-resistant interphases in composite ceramics
This paper considers the problem of heat transfer in a composite ceramic material where the structural elements are bonded to the matrix via a thin heat resistant adhesive layer. The layer has the form of a circular ring or close to it. Using an asymptotic approach, the interphase is modeled by an infinitesimal imperfect interface, preserving the main features of the temperature fields around the interphase, and allowing a significant simplification where FEM analysis is concerned. The nonlinear transmission conditions that accompany such an imperfect interface are evaluated, and their accuracy is verified by means of dedicated analytical examples as well as carefully designed FEM simulations. The interphases of various geometries are analysed, with an emphasis on the influence of the curvature of their boundaries on the accuracy of the evaluated conditions. Numerical results demonstrate the benefits of the approach and its limitations.
1511.06630v2
2015-11-29
Ultrafast electron-phonon-magnon interactions at noble metal-ferromagnet interfaces
Ultrafast optical excitation of gold-cobalt bilayers triggers the nontrivial interplay between the electronic, acoustic, and magnetic degrees of freedom. Laser-heated electrons generated at the gold-air interface diffuse through the layer of gold and strongly overheat the lattice in cobalt resulting in the emission of ultrashort acoustic pulses and generation of exchange-coupled magnons. Time-resolved optical measurements allow for extracting the thermal boundary (Kapitza) resistances at metal/metal interfaces and the hot electron diffusion length in ferromagnetic materials. Both the experimental data and the analytical treatment of the two-temperature model reveal the role of the Kapitza resistance in transient lattice overheating.
1511.09060v3
2016-04-05
Gap state charge induced spin-dependent negative differential resistance in tunnel junctions
We propose and demonstrate through first-principles calculation a new spin-dependent negative differential resistance (NDR) mechanism in magnetic tunnel junctions (MTJ) with cubic cation disordered crystals (CCDC) AlO$_x$ or Mg$_{1-x}$Al$_x$O as barrier materials. The CCDC is a class of insulators whose band gap can be changed by cation doping. The gap becomes arched in an ultrathin layer due to the space charge formed from metal-induced gap states. With an appropriate combination of an arched gap and a bias voltage, NDR can be produced in either spin channel. This mechanism is applicable to 2D and 3D ultrathin junctions with a sufficiently small band gap that forms a large space charge. It provides a new way of controlling the spin-dependent transport in spintronic devices by an electric field. A generalized Simmons formula for tunneling current through junction with an arched gap is derived to show the general conditions under which ultrathin junctions may exhibit NDR.
1604.01364v1
2016-05-12
Thermoelectric performance of spin Seebeck effect in Fe3O4/Pt-based thin film heterostructures
We report a systematic study on the thermoelectric performance of spin Seebeck devices based on Fe3O4/Pt junction systems. We explore two types of device geometries: a spin Hall thermopile and spin Seebeck multilayer structures. The spin Hall thermopile increases the sensitivity of the spin Seebeck effect, while the increase in the sample internal resistance has a detrimental effect on the output power. We found that the spin Seebeck multilayers can overcome this limitation since the multilayers exhibit the enhancement of the thermoelectric voltage and the reduction of the internal resistance simultaneously, therefore resulting in significant power enhancement. This result demonstrates that the multilayer structures are useful for improving the thermoelectric performance of the spin Seebeck effect.
1605.03752v1
2016-06-15
Response of Carbon Nanotube (CNT) Ply Subjected to a Pulsed Magnetic Field
In this study, the possible deformation of a single Carbon Nanotube (CNT) ply subjected to a pulsed magnetic field was investigated. In all tests the capacitor bank was charged to 6kJ of energy. A Photon Doppler Velocimetry (PDV) system was used to measure velocity or displacement of the CNT ply during the experiments. The resistance of the CNT ply was measured using four-point probe technique before and after the experiments. Preliminary results show that the single CNT plies do not permanently deform in response to the pulsed magnetic fields. However, they can be displaced, either by themselves a small amount (0.6mm) or by a large amount using a driver material. Also, the resistance of the CNT plies may increase or decrease depends on the lay-out (i.e., yarn) and current flow directions.
1606.04893v2
2016-07-28
A 3D dislocation dynamics analysis of the size effect on the strength of [111] LiF micropillars at 300K and 600K
The mechanical behavior in compression of [111] LiF micropillars with diameters in the range 0.5 $\mu$m to 2.0 $\mu$m was analyzed by means of discrete dislocation dynamics at ambient and elevated temperature. The dislocation velocity was obtained from the Peach-Koehler force acting on the dislocation segments from a thermally-activated model that accounted for the influence of temperature on the lattice resistance. A size effect of the type "smaller is stronger" was predicted by the simulations, which was in quantitative agreement with previous experimental results by the authors \cite{SWC14}. The contribution of the different physical deformation mechanisms to the size effect (namely, nucleation of dislocations, dislocation exhaustion and forest hardening) could be ascertained from the simulations and the dominant deformation mode could be assessed as a function of the specimen size and temperature. These results shed light into the complex interaction among size, lattice resistance and dislocation mobility in the mechanical behavior of $\mu$m-sized single crystals.
1607.08642v1
2016-11-20
Uniform Benchmarking of Low Voltage Van Der Waals FETs
Monolayer MoS2, MoSe2, MoTe2, WS2, WSe2, and black phosphorous field effect transistors (FETs) operating in the low-voltage (LV) regime (0.3V) with geometries from the 2019 and 2028 nodes of the 2013 International Technology Roadmap for Semiconductors (ITRS) are benchmarked along with an ultra-thin-body Si FET. Current can increase or decrease with scaling, and the trend is strongly correlated with the effective mass. For LV operation at the 2028 node, an effective mass of ~0.4 m0, corresponding to that of WSe2, gives the maximum drive current. The short 6 nm gate length combined with LV operation is forgiving in its requirements for material quality and contact resistances. In this LV regime, device and circuit performance are competitive using currently measured values for mobilities and contact resistances for the monolayer two-dimensional materials.
1611.06480v1
2016-12-28
In-plane anisotropy of transport coefficients in the electronic nematic states: Universal origin of the nematicity in Fe-based superconductors
The origin of the electronic nematicity and its remarkable material-dependence are famous longstanding unsolved issues in Fe-based superconductors. To attack these issues, we focus on the in-plane anisotropy of the resistivity: In the nematic state in FeSe, the relation $\rho_x>\rho_y$ holds, where $\rho_{x(y)}$ is the resistivity along the longer (shorter) Fe-Fe axis. In contrast, the opposite anisotropy $\rho_x<\rho_y$ is realized in other undoped Fe-based superconductors. Such nontrivial material dependence is naturally explained in terms of the strongly orbital-dependent inelastic quasiparticle scattering realized in the orbital-ordered state. The opposite anisotropy between FeSe ($\rho_x>\rho_y$) and other undoped compounds ($\rho_x<\rho_y$) reflects the difference in the number of hole-pockets. We also explain the large in-plane anisotropy of the thermoelectric power in the nematic state.
1612.08841v1
2017-02-03
Evolution of structure, magnetism and electronic transport in doped pyrochlore iridate Y$_2$Ir$_{2-x}$Ru$_{x}$O$_7$
The interplay between spin-orbit coupling (SOC) and electron correlation ($U$) is considered for many exotic phenomena in iridium oxides. We have investigated the evolution of structural, magnetic and electronic properties in pyrochlore iridate Y$_2$Ir$_{2-x}$Ru$_{x}$O$_7$ where the substitution of Ru has been aimed to tune this interplay. The Ru substitution does not introduce any structural phase transition, however, we do observe an evolution of lattice parameters with the doping level $x$. X-ray photoemission spectroscopy (XPS) study indicates Ru adopts charge state of Ru$^{4+}$ and replaces the Ir$^{4+}$ accordingly. Magnetization data reveal both the onset of magnetic irreversibility and the magnetic moment decreases with progressive substitution of Ru. These materials show non-equilibrium low temperature magnetic state as revealed by magnetic relaxation data. Interestingly, we find magnetic relaxation rate increases with substitution of Ru. The electrical resistivity shows an insulating behavior in whole temperature range, however, resistivity decreases with substitution of Ru. Nature of electronic conduction has been found to follow power-law behavior for all the materials.
1702.01023v1
2017-02-25
Compressive mechanical response of graphene foams and their thermal resistance with copper interfaces
We report compressive mechanical response of graphene foams (GFs) and the thermal resistance ($R_{TIM}$) between copper (Cu) and GFs, where GFs were prepared by the chemical vapor deposition (CVD) method. We observe that Young's modulus ($E_{GF}$) and compressive strength ($\sigma_{GF}$) of GFs have a power law dependence on increasing density ($\rho_{GF}$) of GFs. The maximum efficiency of absorbed energy ($\eta_{max}$) for all GFs during the compression is larger than ~0.39. We also find that a GF with a higher $\rho_{GF}$ shows a larger $\eta_{max}$. In addition, we observe that the measured $R_{TIM}$ of Cu/GFs at room temperature with a contact pressure of 0.25 MP applied increases from ~50 to ~90 $mm^2K/W$ when $\rho_{GF}$ increases from 4.7 to 31.9 $mg/cm^3$.
1702.07816v1
2017-11-22
Structural properties of Fe/Cu magnetic multilayers: a Monte Carlo approach
Using atomistic Monte Carlo simulations, we investigated the impact of the interface on the structural properties of iron and copper (Fe/Cu) magnetic multilayers grown by Vorono\"i diagram. Interest in magnetic multilayers has recently emerged as they are shown to be promising candidates for magnetic storage media, magneto-resistive sensors, and personalized medical treatment. As these artificial materials show large differences in properties compared to conventional ones, many experimental and theoretical works have been dedicated on shedding light on these differences and tremendous results have emerged. However, little is known how the interfaces influence the structure of the layers around them. By a numerical approach, we show that the structure of each layer depends on its thickness and the interface morphology. The Fe and Cu layers can adopt either the body-centered-cubic (bcc) or face-centered-cubic (fcc) structure, while the interface can assume amorphous, bcc, fcc, or a mixture of bcc and fcc structures depending on the layer thicknesses. These results are in good agreement with the experiments. They could be helpful in understanding effects such as giant magneto-resistance from the structural viewpoint.
1711.08508v1
2017-11-24
Inter-layer and Intra-layer Heat Transfer in Bilayer/Monolayer Graphene van der Waals Heterostructure: Is There a Kapitza Resistance Analogous?
Van der Waals heterostructures have exhibited interesting physical properties. In this paper, heat transfer in hybrid coplanar bilayer/monolayer (BL-ML) graphene, as a model layered van der Waals heterostructure, was studied using non-equilibrium molecular dynamics (MD) simulations. Temperature profile and inter- and intra-layer heat fluxes of the BL-ML graphene indicated that, there is no fully developed thermal equilibrium between layers and the drop in average temperature profile at the step-like BL-ML interface is not attributable to the effect of Kapitza resistance. By increasing the length of the system up to 1 $\mu$m in the studied MD simulations, the thermally non-equilibrium region was reduced to a small area near the step-like interface. All MD results were compared to a continuum model and a good match was observed between the two approaches. Our results provide a useful understanding of heat transfer in nano- and micro-scale layered 2D materials and van der Waals heterostructures.
1711.09127v1
2018-04-20
Comparative study of the compensated semi-metals LaBi and LuBi : A first-principles approach
We have investigated the electronic structures of LaBi and LuBi, employing the full-potential all electron method as implemented in Wien2k. Using this, we have studied in detail both the bulk and the surface states of these materials. From our band structure calculations we find that LuBi, like LaBi, is a compensated semi-metal with almost equal and sizable electron and hole pockets. In analogy with experimental evidence in LaBi, we thus predict that LuBi will also be a candidate for extremely large magneto-resistance (XMR), which should be of immense technological interest. Our calculations reveal that LaBi, despite being gapless in the bulk spectrum, displays the characteristic features of a $\mathbb{Z}_{2}$ topological semi-metal, resulting in gapless Dirac cones on the surface, whereas LuBi only shows avoided band inversion in the bulk and is thus a conventional compensated semi-metal with extremely large magneto-resistance.
1804.07652v1
2014-08-02
Destroyed quantum Hall effect in graphene with [0001] tilt grain boundaries
The reason why the half-integer quantum Hall effect (QHE) is suppressed in graphene grown by chemical vapor deposition (CVD) is unclear. We propose that it might be connected to extended defects in the material and present results for the quantum Hall effect in graphene with [0001] tilt grain boundaries connecting opposite sides of Hall bar devices. Such grain boundaries contain 5-7 ring complexes that host defect states that hybridize to form bands with varying degree of metallicity depending on grain boundary defect density. In a magnetic field, edge states on opposite sides of the Hall bar can be connected by the defect states along the grain boundary. This destroys Hall resistance quantization and leads to non-zero longitudinal resistance. Anderson disorder can partly recover quantization, where current instead flows along returning paths along the grain boundary depending on defect density in the grain boundary and on disorder strength. Since grain sizes in graphene made by chemical vapor deposition are usually small, this may help explain why the quantum Hall effect is usually poorly developed in devices made of this material.
1408.0394v1
2019-02-21
Correlation in transport coefficients of hole-doped CuRhO$_2$ single crystals
To clarify the origin of the nontrivial thermoelectric properties observed in the delafossite oxide CuRhO$_2$ polycrystals, we have performed the systematic transport measurements on the single-crystalline CuRhO$_2$ samples. In the parent compound, we find a pronounced peak structure due to a phonon-drag effect in the temperature dependence of the Seebeck coefficient, which is also confirmed by the size effect experiments. In the Mg-substituted crystals, in contrast to the results of the polycrystals, both the resistivity and the Seebeck coefficient decrease with increasing Mg content $y$. In particular, the coefficient $A$ for the $T^2$ term of the resistivity and the $T$-linear coefficient for the Seebeck coefficient at low temperatures are well described within a simple relationship expected for metals, which is also applicable to the correlated materials with low carrier densities.
1902.08301v1
2020-04-14
Temperature overshoot as the cause of physical changes in resistive switching devices during electro-formation
Resistive switching devices based on transition metal oxides require formation of a conductive filament in order for the device to be able to switch. Such filaments have been proposed to form by the reduction of the oxide due to application of the electric field, but this report seeks to rebut that interpretation. Frequently reported physical changes during electro-formation include delamination of electrodes, crystallization of functional oxide, intermixing of electrode and oxide materials, and extensive loss of oxygen presumably to the ambient. Here we show that most of these effects are not inherent to the formation and switching processes and instead are due to an experimental artifact: the discharge of parasitic capacitances in the forming circuit. Discharge of typical BNC cables can raise the temperature of the filament to between 2,000 and 5,000 K resulting in extensive physical changes. Discharge and associated effects mentioned above can be eliminated using an on-chip load element without affecting the ability to switch.
2004.06571v1
2020-09-04
Effective Thermal Conductivity of SrBi$_4$Ti$_4$O$_{15}$-La$_{0.7}$Sr$_{0.3}$MnO$_3$ Oxide composite: Role of Particle Size and Interface Thermal Resistance
We present a novel approach to reduce the thermal conductivity ($\kappa$) in thermoelectric composite materials using acoustic impedance mismatch and the Debye model. Also, the correlation between interface thermal resistance (R$_{int}$) and the particle size of the dispersed phase on the k of the composite is discussed. In particular, the $\kappa$ of an oxide composite which consists of a natural superlattice Aurivillius phase (SrBi$_4$Ti$_4$O$_{15}$) as a matrix and perovskite (La$_{0.7}$Sr$_{0.3}$MnO$_3$) as a dispersed phase is investigated. A significant reduction in the $\kappa$ of composite, even lower than the $\kappa$ of the matrix when the particle size of La$_{0.7}$Sr$_{0.3}$MnO$_3$ is smaller than the Kapitza radius (a$_K$) is observed, depicting that R$_{int}$ dominates for particle size lower than a$_K$ due to increased surface to volume ratio. The obtained results have the potential to provide new directions for engineering composite thermoelectric systems with desired thermal conductivity and promising in the field of energy harvesting.
2009.02218v1
2022-02-25
Low-Temperature Thermal Conductivity of CeRh$_{2}$As$_{2}$
CeRh$_2$As$_2$ is a rare unconventional superconductor ($T_c=0.26$ K) characterized by two adjacent superconducting phases for a magnetic field $H \parallel c$-axis of the tetragonal crystal structure. Antiferromagnetic order, quadrupole-density-wave order ($T_0 = 0.4$ K) and the proximity of this material to a quantum-critical point have also been reported: The coexistence of these phenomena with superconductivity is currently under discussion. Here, we present thermal conductivity and electrical resistivity measurements on a single crystal of CeRh$_2$As$_2$ between 60 mK and 200 K and in magnetic fields ($H \parallel c$) up to 8 T. Our measurements at low $T$ verify the Wiedemann-Franz law within the error bars. The $T$ dependence of the thermal conductivity $\kappa(T)$ shows a pronounced drop below $T_c$ which is also field dependent and thus interpreted as the signature of superconductivity. However, the large residual resistivity and the lack of sharp anomalies in $\kappa(T)$ at the expected transition temperatures clearly indicate that samples of much higher purity are required to gain more information about the superconducting gap structure.
2202.12667v1
2016-03-07
Pressure-resistant intermediate valence in Kondo insulator SmB6
Resonant x-ray emission spectroscopy (RXES) was used to determine the pressure dependence of the f-electron occupancy in the Kondo insulator SmB6. Applied pressure reduces the f-occupancy, but surprisingly, the material maintains a significant divalent character up to a pressure of at least 35 GPa. Thus, the closure of the resistive activation energy gap and onset of magnetic order are not driven by stabilization of an integer valent state. Over the entire pressure range, the material maintains a remarkably stable intermediate valence that can in principle support a nontrivial band structure.
1603.02207v1
2017-04-01
Small-signal model for 2D-material based field-effect transistors targeting radio-frequency applications: the importance of considering non-reciprocal capacitances
A small-signal equivalent circuit of 2D-material based field-effect transistors is presented. Charge conservation and non-reciprocal capacitances have been assumed so the model can be used to make reliable predictions at both device and circuit levels. In this context, explicit and exact analytical expressions of the main radio-frequency figures of merit of these devices are given. Moreover, a direct parameter extraction methodology is provided based on S-parameter measurements. In addition to the intrinsic capacitances, transconductance and output conductance, our approach allows extracting the series combination of drain/source metal contact and access resistances. Accounting for these extrinsic resistances is of upmost importance when dealing with low dimensional field-effect transistors.
1704.00181v2
2017-04-05
An open-source platform to study uniaxial stress effects on nanoscale devices
We present an automatic measurement platform that enables the characterization of nanodevices by electrical transport and optical spectroscopy as a function of uniaxial stress. We provide insights into and detailed descriptions of the mechanical device, the substrate design and fabrication, and the instrument control software, which is provided under open-source license. The capability of the platform is demonstrated by characterizing the piezo-resistance of an InAs nanowire device using a combination of electrical transport and Raman spectroscopy. The advantages of this measurement platform are highlighted by comparison with state-of-the-art piezo-resistance measurements in InAs nanowires. We envision that the systematic application of this methodology will provide new insights into the physics of nanoscale devices and novel materials for electronics, and thus contribute to the assessment of the potential of strain as a technology booster for nanoscale electronics.
1704.01394v1
2017-08-09
Contact-Induced Semiconductor-to-Metal Transition in Single-Layer WS$_2$
Low-resistance ohmic contacts are a challenge for electronic devices based on two-dimensional materials. We show that an atomically precise junction between a two-dimensional semiconductor and a metallic contact can lead to a semiconductor-to-metal transition in the two-dimensional material--a finding which points the way to a possible method of achieving low-resistance junctions. Specifically, single-layer WS$_2$ undergoes a semiconductor-to-metal transition when epitaxially grown on Ag(111), while it remains a direct band gap semiconductor on Au(111). The metallicity of the single layer on Ag(111) is established by lineshape analysis of core level photoemission spectra. Angle-resolved photoemission spectroscopy locates the metallic states near the Q point of the WS$_2$ Brillouin zone. Density functional theory calculations show that the metallic states arise from hybridization between Ag bulk bands and the local conduction band minimum of WS$_2$ near the Q point.
1708.02799v1
2019-08-26
Local electrodynamics of a disordered conductor model system measured with a microwave impedance microscope
We study the electrodynamic impedance of percolating conductors with a pre-defined network topology using a scanning microwave impedance microscope (sMIM) at GHz frequencies. For a given percolation number we observe strong spatial variations across a sample which correlate with the connected regions (clusters) in the network when the resistivity is low such as in Aluminum. For the more resistive material NbTiN the impedance becomes dominated by the local structure of the percolating network (connectivity). The results can qualitatively be understood and reproduced with a network current spreading model based on the pseudo-inverse Laplacian of the underlying network graph.
1908.09810v1
2019-11-30
Structural relaxation in amorphous materials under cyclic tension-compression loading
The process of structural relaxation in disordered solids subjected to repeated tension-compression loading is studied using molecular dynamics simulations. The binary glass is prepared by rapid cooling well below the glass transition temperature and then periodically strained at constant volume. We find that the amorphous system is relocated to progressively lower potential energy states during hundreds of cycles, and the energy levels become deeper upon approaching critical strain amplitude from below. The decrease in potential energy is associated with collective nonaffine rearrangements of atoms, and their rescaled probability distribution becomes independent of the cycle number at sufficiently large time intervals. It is also shown that yielding during startup shear deformation occurs at larger values of the stress overshoot in samples that were cyclically loaded at higher strain amplitudes. These results might be useful for mechanical processing of amorphous alloys in order to reduce their energy and increase chemical resistivity and resistance to crystallization.
1912.00221v1
2021-01-04
Twin Mechanical Metamaterials
By mimicking the geometrical relation of nano-twin crystals, we propose novel architected twin mechanical metamaterials (TMMs), which can impede local shearing band formation under external loading, thus avoiding global catastrophic failure. The effects of twin-space and twin angle on the mechanical performance of TMMs were also explored, such as: energy absorption, strength, and crack propagation resistance. The results showed that the twin topology design can not only significantly improve the energy-absorption efficiency but also remarkably improve the crack-propagation resistances of stretching-dominant mechanical metamaterials. We also studied the effect of twin-space and twin angle on the tensile strength of TMMs. This study is the first to report on the inverse Hall-Petch effect of TMMs. Our findings open an avenue for the design and fabrication of advanced materials with exceptionally tuneable mechanical properties.
2101.00927v1
2012-06-04
Optimal Condition for Strong Terahertz Radiation from Intrinsic Josephson Junctions
In order to enhance the radiation power in terahertz band based on the intrinsic Josephson junctions of Bi$_2$Sr$_2$CaCu$_2$O$_{8+\delta}$ single crystal, we investigate a long cylindrical sample embedded in a dielectric material. Tuning the dielectric constant, the radiation power has a maximum which is achieved when it equals the dissipation caused by Josephson plasma. This yields the optimal dielectric constant of wrapping material in terms of the properties of BSCCO single crystal. The maximal radiation power is found proportional to the product of the typical superconducting current squared and the typical normal resistance, or the gap energy squared divided by the typical normal resistance, which offers a guideline for choosing superconductor as a source of strong radiation. By introducing an anti-reflection layer, we can build a compact device with the BSCCO cylinder and two wrapping dielectric layers with finite thicknesses.
1206.0516v1
2012-06-15
Breakdown of the interlayer coherence in twisted bilayer graphene
Coherent motion of the electrons in the Bloch states is one of the fundamental concepts of the charge conduction in solid state physics. In layered materials, however, such a condition often breaks down for the interlayer conduction, when the interlayer coupling is significantly reduced by e.g. large interlayer separation. We report that complete suppression of coherent conduction is realized even in an atomic length scale of layer separation in twisted bilayer graphene. The interlayer resistivity of twisted bilayer graphene is much higher than the c-axis resistivity of Bernal-stacked graphite, and exhibits strong dependence on temperature as well as on external electric fields. These results suggest that the graphene layers are significantly decoupled by rotation and incoherent conduction is a main transport channel between the layers of twisted bilayer graphene.
1206.3410v1
2015-07-23
Electronic, magnetic and transport properties of Fe intercalated 2H-TaS$_2$ studied by means of the KKR-CPA method
The electronic, magnetic and transport properties of Fe intercalated 2H-TaS$_2$ have been investigated by means of the Korringa-Kohn-Rostoker (KKR) method. The non-stoichiometry and disorder in the system has been accounted for using the Coherent Potential Approximation (CPA) alloy theory. A pronounced influence of disorder on the spin magnetic moment has been found for the ferro-magnetically ordered material. The same applies for the spin-orbit induced orbital magnetic moment and magneto-crystalline anisotropy energy. The temperature-dependence of the resistivity of disordered 2H-Fe$_{0.28}$TaS$_2$ investigated on the basis of the Kubo-St\v{r}eda formalism in combination with the alloy analogy model has been found in very satisfying agreement with experimental data. This also holds for the temperature dependent anomalous Hall resistivity $ \rho_{\rm xy}(T) $. The role of thermally induced lattice vibrations and spin fluctuations for the transport properties is discussed in detail.
1507.06544v1
2018-07-18
Thermoelectric stack sample cooling modification of a commercial atomic force microscopy
Enabling temperature dependent experiments in Atomic Force Microscopy is of great interest to study materials and surface properties at the nanoscale. By studying Curie temperature of multiferroic materials, temperature based phase transition on crystalline structures or resistive switching phenomena are only a few examples of applications. We present an equipment capable of cooling samples using a thermoelectric cooling stage down to -61.4 C in a 15x15 mm sample plate. The equipment uses a four-unit thermoelectric stack to achieve maximum temperature range, with low electrical and mechanical noise. The equipment is installed into a Keysight 5500LS Atomic Force Microscopy maintaining its compatibility with all Electrical and Mechanical modes of operation. We study the contribution of the liquid cooling pump vibration into the cantilever static deflection noise and the temperature dependence of the cantilever deflection. A La0.7Sr0.3MnO3-y thin film sample is used to demonstrate the performance of the equipment and its usability by analysing the resistive switching phenomena associated with this oxide perovskite.
1807.06876v1
2019-01-21
Ferromagnetic Kondo lattice behavior in Ce11Pd4In9
We report on the low-temperature physical properties of a novel compound Ce$_{11}$Pd$_4$In$_9$ that crystallizes with the orthorhombic Nd$_{11}$Pd$_4$In$_9$-type crystal structure (space group $Cmmm$). The compound exhibits ferromagnetic ordering at $T_{\rm {C}}$ = 18.6 K and an order-order transition at $T_{\rm {t}}$ $\sim$~1.6 K, as inferred from the low-temperature magnetic susceptibility, heat capacity and electrical resistivity data. In the paramagnetic region, the electrical transport in Ce$_{11}$Pd$_4$In$_9$ is dominated by Kondo effect. Below $T_{\rm {C}}$, a distinct contribution due to ferromagnetic spin waves dominates the electrical resistivity data, while at the lowest temperatures, the electrical transport and thermodynamic properties are governed by strong electron-electron correlations. The features observed conjointly hint at strongly correlated ground state in Ce$_{11}$Pd$_4$In$_9$ .
1901.06888v1
2019-11-14
Absence of evidence of spin transport through amorphous Y$_3$Fe$_5$O$_{12}$
Long-distance transport of spin information in insulators without long-range magnetic order has been recently reported. Here, we perform a complete characterization of amorphous Y$_3$Fe$_5$O$_{12}$ (a-YIG) films grown on top of SiO$_2$. We confirm a clear amorphous structure and paramagnetic behavior of our a-YIG films, with semiconducting behavior resistivity that strongly decays with increasing temperature. The non-local transport measurements show a signal which is not compatible with spin transport and can be attributed to the drop of the a-YIG resistivity caused by Joule heating. Our results emphasize that exploring spin transport in amorphous materials requires careful procedures in order to exclude the charge contribution from the spin transport signals.
1911.06061v2
2019-11-15
Design and Performance of Hafnium Optical and Near-IR Kinetic Inductance Detectors
We report on the design and performance of Microwave Kinetic Inductance Detectors (MKIDs) sensitive to single photons in the optical to near-infrared range using hafnium as the sensor material. Our test device had a superconducting transition temperature of 395 mK and a room temperature normal state resistivity of 97 $\mu \Omega$ cm with an RRR = 1.6. Resonators on the device displayed internal quality factors of around 200,000. Similar to the analysis of MKIDs made from other highly resistive superconductors, we find that modeling the temperature response of the detector requires an extra broadening parameter in the superconducting density of states. Finally, we show that this material and design is compatible with a full-array fabrication process which resulted in pixels with decay times of about 40 $\mu$s and resolving powers of ~9 at 800 nm.
1911.06434v1
2020-01-08
Effect of memory electrical switching in metal/vanadium oxide/silicon structures with VO2 films obtained by the sol-gel method
Electrical switching and rectifying properties of the metal-VO2-Si structures, on both p-type and n-type silicon, with vanadium dioxide films obtained by an acetylacetonate sol-gel method, are studied. The switching effect is shown to be due to the semiconductor-to-metal phase transition (SMPT) in vanadium dioxide. The shift of the switching threshold voltage, accompanied by the memory effect, in forward bias of the p-Si-VO2 anisotype heterojunction is observed. To explain this effect, a model is proposed which suggests the existence of an additional series resistance associated with a channel at the VO2/Si interface, where a SiOx layer forms during the VO2 deposition process. This resistance is responsible for both threshold switching characteristics, and the memory effect, and the oxygen ion electromigration process is shown to underlie this effect. Potential applications of the observed phenomena, combining the effects of ReRAM and SMPT, in oxide electronics are discussed.
2001.03055v1
2020-05-24
Schottky barriers, emission regimes and contact resistances in 2H-1T' MoS$_2$ lateral metal-semiconductor junctions from first-principles
We have studied the finite bias transport properties of a 2H-1T' MoS$_2$ lateral metal-semiconductor (M-S) junction by non-equilibrium Green's functions calculations, aimed at contacting the 2D channel in a field effect transistor. Our results indicate that (a) despite the fundamentally different electrostatics of line and planar dipoles, the Schottky barrier heights respond similarly to changes in doping and applied bias in 2D and 3D M-S junctions, (b) 2H-1T' MoS$_2$ lateral junctions are free from Fermi level pinning, (c) armchair interfaces have superior contacting properties vs.\ zigzag interfaces, (d) 1T' contacts to $p$ channels will present a reduced contact resistance by a factor of 4-10 with respect to $n$ channels and (e) contacts to intermediately doped $n$ ($p$) channels operate in the field (thermionic) emission regime. We also provide an improved procedure to experimentally determine the emission regime in 2D material junctions.
2005.11717v1
2020-06-12
Blocking of conducting channels widens window for ferroelectric resistive switching in interface-engineered Hf0.5Zr0.5O2 tunnel devices
Films of Hf0.5Z0.5O2 (HZO) contain a network of grain boundaries. In (111) HZO epitaxial films on (001) SrTiO3, for instance, twinned orthorhombic (o-HZO) ferroelectric crystallites coexist with grain boundaries between o-HZO and a residual paraelectric monoclinic (m-HZO) phase. These grain boundaries contribute to the resistive switching response in addition to the genuine ferroelectric polarization switching and have detrimental effects on device performance. Here, it is shown that, by using suitable nanometric capping layers deposited on HZO film, a radical improvement of the operation window of the tunnel device can be achieved. Crystalline SrTiO3 and amorphous AlOx are explored as capping layers. It is observed that these layers conformally coat the HZO surface and allow to increase the yield and homogeneity of functioning ferroelectric junctions while strengthening endurance. Data show that the capping layers block ionic-like transport channels across grain boundaries. It is suggested that they act as oxygen suppliers to the oxygen-getters grain boundaries in HZO. In this scenario it could be envisaged that these and other oxides could also be explored and tested for fully compatible CMOS technologies.
2006.07048v1
2020-07-09
Fe3Se4: A Possible Ferrimagnetic Half-Metal?
Half-metallic ferromagnets show 100% spin-polarization at the Fermi level and are ideal candidates for spintronic applications. Despite the extensive research in the field, very few materials have been discovered so far. Here we present results of electronic band structure calculations based on density functional theory and extensive physical-property measurements for Fe3Se4 revealing signatures of half-metallicity. The spin-polarized electronic band structure calculations predict half-metallic ferrimagnetism for Fe3Se4. The electrical resistivity follows exponentially suppressed electron-magnon scattering mechanism in the low-temperature regime and show a magnetoresistance effect that changes the sign from negative to positive with decreasing temperature around 100 K. Other intriguing observations include the anomalous behavior of Hall resistance below 100 K and an anomalous Hall coefficient that roughly follows the \r{ho}2 behavior.
2007.04736v1
2020-07-29
Quasiparticle and Nonquasiparticle Transport in Doped Quantum Paraelectrics
Charge transport in doped quantum paralectrics (QPs) presents a number of puzzles, including a pronounced $T^2$ regime in the resistivity. We analyze charge transport in a QP within a model of electrons coupled to a soft transverse optical (TO) mode via a two-phonon mechanism. For $T$ above the soft-mode frequency but below some characteristic scale ($E_0$), the resistivity scales with the occupation number of phonons squared, i.e., as $T^2$. The $T^2$ scattering rate does not depend on the carrier number density and is not affected by a crossover between degenerate and non-degenerate regimes, in agreement with the experiment. Temperatures higher than $E_0$ correspond to a non-quasiparticle regime, which we analyze by mapping the Dyson equation onto a problem of supersymmetric quantum mechanics. The combination of scattering by two TO phonons and by a longitudinal optical mode explains the data quite well.
2007.14947v2
2020-08-06
Magnetic, transport, and thermal properties of $δ$-phase UZr$_2$
Alloys of hexagonal $\delta$-phase UZr$_2$ have been synthesized and studied by means of heat capacity, magnetic susceptibility, magnetization, electrical resistivity, magnetoresistance, thermoelectric power, thermal conductivity measurements, for the first time, at temperatures from 1.8 to 300 K and in magnetic fields up to 8 T. The weak temperature dependence of the magnetic susceptibility and the small value of both Seebeck (0.75 $\mu$V/K at room temperature) and of the Sommerfeld coefficient (13.5 mJ mol$^{-1}$ K$^{-2}$) point to 5$f$-electrons in this material having a delocalized nature. The electrical resistivity and magnetoresistance indicate the presence of significant electronic disorder in $\delta$-UZr$_2$, consistent with the disorder in its crystal structure. Density functional theory calculations have been performed and compared to experimental results.
2008.02746v1
2020-12-29
Magnetotransport signatures of chiral magnetic anomaly in the half-Heusler phase ScPtBi
Study of magnetotransport properties of ScPtBi revealed simultaneously: a negative contribution to the longitudinal magnetoresistance, the planar Hall effect, and distinct angular narrowing of the longitudinal magnetoresistance { three hallmarks of chiral magnetic anomaly (pumping of axial charge between Weyl nodes), a distinct property of topological semimetals. Electronic structure calculations show that structural defects, such as antisites and vacancies, bring substantial density of states at the Fermi level of ScPtBi, indicating that it is a semimetal, not a zero-gap semiconductor, as predicted earlier. This is in accord with electrical resistivity in ScPtBi, showing no characteristics of semiconductor. Moreover, below 0.7K we observed an onset of a superconducting transition, with the resistivity disappearing completely below 0.23 K.
2012.14819v2
2021-05-28
Projected mushroom-type phase-change memory
Phase-change memory devices have found applications in in-memory computing where the physical attributes of these devices are exploited to compute in place without the need to shuttle data between memory and processing units. However, non-idealities such as temporal variations in the electrical resistance have a detrimental impact on the achievable computational precision. To address this, a promising approach is projecting the phase configuration of phase change material onto some stable element within the device. Here we investigate the projection mechanism in a prominent phase-change memory device architecture, namely mushroom-type phase-change memory. Using nanoscale projected Ge2Sb2Te5 devices we study the key attributes of state-dependent resistance, drift coefficients, and phase configurations, and using them reveal how these devices fundamentally work.
2105.13693v2
2021-08-04
Current-induced breakdown of the quantum anomalous Hall effect
The quantum anomalous Hall effect (QAHE) realizes dissipationless longitudinal resistivity and quantized Hall resistance without the need of an external magnetic field. However, when reducing the device dimensions or increasing the current density, an abrupt breakdown of the dissipationless state occurs with a relatively small critical current, limiting the applications of the QAHE. We investigate the mechanism of this breakdown by studying multi-terminal devices and identified that the electric field created between opposing chiral edge states lies at the origin. We propose that electric-field-driven percolation of two-dimensional charge puddles in the gapped surface states of compensated topological-insulator films is the most likely cause of the breakdown.
2108.02081v1
2021-10-08
Universal Non-Volatile Resistive Switching Behavior in 2D Metal Dichalcogenides Featuring Unique Conductive-Point Random Access Memory Effect
Two-dimensional materials have been discovered to exhibit non-volatile resistive switching (NVRS) phenomenon. In our work, we reported the universal NVRS behavior in a dozen metal dichalcogenides, featuring low switching voltage, large on/off ratio, fast switching speed and forming free characteristics. A unique conductive-point random access memory (CPRAM) effect is used to explain the switching mechanisms, supported by experimental results from current-sweep measurements.
2110.03863v1
2021-10-27
Bound on resistivity in flat-band materials due to the quantum metric
The quantum metric is a central quantity of band theory but has so far not been related to many response coefficients due to its nonclassical origin. However, within a newly developed Kubo formalism for fast relaxation, the decomposition of the dc electrical conductivity into both classical (intraband) and quantum (interband) contributions recently revealed that the interband part is proportional to the quantum metric. Here, we show that interband effects due to the quantum metric can be significantly enhanced and even dominate the conductivity for semimetals at charge neutrality and for systems with highly quenched bandwidth. This is true in particular for topological flat-band materials of nonzero Chern number, where for intermediate relaxation rates an upper bound exists for the resistivity due to the common geometrical origin of quantum metric and Berry curvature. We suggest to search for these effects in highly tunable rhombohedral trilayer graphene flakes.
2110.14658v3
2021-11-22
First-principles-based screening method for resistivity scaling of anisotropic metals
The resistivity scaling of metals is a crucial limiting factor for further downscaling of interconnects in nanoelectronic devices that affects signal delay, heat production, and energy consumption. Here, we generalize a commonly considered figure of merit for selecting promising candidate metals with highly anisotropic Fermi surfaces in terms of their electronic transport properties at the nanoscale. For this, we introduce a finite-temperature transport tensor, based on band structures obtained from first principles. This transport tensor allows for a straightforward comparison between highly anisotropic metals in nanostructures with different lattice orientations and arbitrary transport directions. By evaluating the temperature dependence of the tensor components, we also assess the validity of a Fermi surface-based evaluation of the transport properties at zero temperature, rather than considering standard operating temperature conditions.
2111.11121v2
2021-12-17
Nanoscale laser flash measurements of diffuson transport in amorphous Ge and Si
The thermal properties of amorphous materials have attracted significant attention due to their technological importance in electronic devices. Additionally, the disorder-induced breakdown of the phonon gas model makes vibrational transport in amorphous materials a topic of fundamental interest. In the past few decades, theoretical concepts such as propagons, diffusons, and locons have emerged to describe different types of vibrational modes in disordered solids. But experiments can struggle to accurately determine which types of vibrational states carry the majority of the heat. In the present study, we use nanoscale laser flash measurements (front/back time-domain thermoreflectance) to investigate thermal transport mechanisms in amorphous Ge and amorphous Si thin-films. We observe a nearly linear relationship between the amorphous film's thermal resistance and the film's thickness. The slope of the film's thermal resistance vs. thickness corresponds to a thickness-independent thermal conductivity of 0.4 and 0.6 W/(m-K) for a-Ge and a-Si, respectively. This result reveals that the majority of heat currents in amorphous Si and Ge thin films prepared via RF sputtering at room temperature are carried by diffusons and/or propagons with mean free paths less than a few nanometers.
2112.09289v2
2022-01-06
Insights to negative differential resistance in \texorpdfstring{MoS\textsubscript{2}}{MoS2} Esaki diodes: a first-principles perspective
\ce{MoS_2} is a two dimensional material with a band gap depending on the number of layers and tunable by an external electric field. The experimentally observed intralayer band-to-band tunneling and interlayer band-to-band tunneling in this material present an opportunity for new electronic applications in tunnel field effect transistors. However, such a widely accepted concept has never been supported up by theoretical investigations based on first principles. In this work, using density functional theory, in conjunction with non-equilibrilibrium Green's function techniques and our electric field gating method, enabled by a large-scale computational approach, we study the relation between band alignment and transmission in planar and side-stack \ce{MoS_2} $p$-$i$-$n$ junction configurations. We demonstrate the presence of negative differential resistance for both in-plane and interlayer current, a staple characteristic of tunnel diode junctions, and analyze the physical origin of such an effect. Electrostatic potentials, the van der Waals barrier, and complex band analysis are also examined for a thorough understanding of Esaki Diodes.
2201.02178v1
2022-05-21
Increased Phase Coherence Length in a Porous Topological Insulator
The surface area of Bi2Te3 thin films was increased by introducing nanoscale porosity. Temperature dependent resistivity and magnetotransport measurements were conducted both on as-grown and porous samples (23 and 70 nm). The longitudinal resistivity of the porous samples became more metallic, indicating the increased surface area resulted in transport that was more surface-like. Weak antilocalization (WAL) was present in all samples, and remarkably the phase coherence length doubled in the porous samples. This increase is likely due to the large Fermi velocity of the Dirac surface states. Our results show that the introduction of nanoporosity does not destroy the topological surface states but rather enhances them, making these nanostructured materials promising for low energy electronics, spintronics and thermoelectrics.
2205.10589v1
2022-07-11
Spin-Orbit Proximity Effect in Bi/Co Multilayer: The Role of Interface Scattering
The Spin-Orbit Proximity Effect is the raise of Spin-Orbit Coupling at a layer near to the interface with a strong spin-orbit material. It has been seen in several system such as graphene and ferromagnetic layers. The control of the Spin-Orbit Coupling can be a pathway to discover novel and exotic phases in superconductor and semimetallic systems. Here, we study the magnetoelectrical transport, i.e., magnetoresistance and anomalous Hall effect, in Cobalt/Bismuth multilayers looking for traces of spin-orbit proximity effect and evaluate the origin of such effect. Our results point for an increase of Spontaneous Magnetic Anisotropy of Resistivity and Anomalous Hall Resistivity at very low thicknesses of Cobalt. The analysis of the Anomalous Hall Resisitivity indicate that the Bismuth layers change the scattering mechanism of Hall effect to the extrinsic skew-scattering type, indicating that the spin-orbit proximity effect could be related to the elastic scattering of cobalt free carriers by bismuth sites at the interface.
2207.04937v1
2022-08-22
Unified intermediate coupling description of the pseudogap and the strange metal phases of cuprates
A one band Hubbard model with intermediate coupling is shown to describe the two most important unusual features of a normal state: linear resistivity strange metal and the pseudogap. Both the spectroscopic and transport properties of the cuprates are considered on the same footing by employing a relatively simple postgaussian approximation valid for the intermediate couplings $U/t=1.5-4$ in relevant temperatures $T>100{\rm K}.$ In the doping range $\ p=0.1-0.3$, the value of $U$ is smaller than that in the parent material. For a smaller doping, especially in the Mott insulator phase, the coupling is large compared to the effective tight binding scale and a different method is required. This scenario provides an alternative to the paradigm that the coupling should be strong, say $U/t>6$, in order to describe the strange metal. We argue that to obtain phenomenologically acceptable underdoped normal state characteristics like $T^{\ast }$, pseudogap values, and spectral weight distribution, a large value of $U$ is detrimental. Surprisingly the resistivity in the above temperature range is linear $\rho =\rho_{0}+\alpha \frac{m^{\ast }}{e^{2}n\hbar }T$ with the "Planckian" coefficient $\alpha $ of order one.
2208.10093v1
2022-09-05
Charge-Density Wave Driven Giant Thermionic-Current Switching in 1T-TaS$_{2}$/2H-TaSe$_{2}$/2H-MoS$_{2}$ Heterostructure
1T-TaS$_2$ exhibits several resistivity phases due to the modulation of charge density wave (CDW). The fact that such phase transition can be driven electrically has attracted a lot of attention in the recent past towards \emph{active-metal} based electronics. However, the bias-driven resistivity switching is not very large ($<$ 5 fold), and an enhancement in the same will highly impact such phase transition devices. One aspect that is often overlooked is that such phase transition is also accompanied by a significant change in the local temperature due to the low thermal conductivity of 1T-TaS$_2$. In this work, we exploit such electrically driven phase transition induced temperature change to promote carriers over a thermionic barrier in a 1T-TaS$_{2}$/2H-TaSe$_{2}$/2H-MoS$_{2}$ T-Junction, achieving a $964$-fold abrupt switching in the current through the MoS$_2$ channel. The device is highly reconfigurable and exhibits an abrupt reduction in current as well when the biasing configuration changes. The results are promising for several electronic applications, including neuromorphic chips, switching, nonlinear devices, and industrial electronics such as current and temperature sensing.
2209.02024v1
2022-11-18
Pressure-induced superconductivity in PdTeI with quasi-one-dimensional PdTe chains
The quasi-one-dimensional material PdTeI exhibits unusual electronic transport properties at ambient pressure. Here, we systematically investigate both the structural and electronic responses of PdTeI to external pressure, through a combination of electrical transport, synchrotron x-ray diffraction (XRD), and Raman spectroscopy measurements. The charge density wave (CDW) order in PdTeI is fragile and the transition temperature TCDW decreases rapidly with the application of external pressure. The resistivity hump is indiscernible when the pressure is increased to 1 GPa. Upon further compression, zero resistance is established above 20 GPa, suggesting the occurrence of superconductivity. Combined XRD and Raman data evidence that the emergence of superconductivity is accompanied by a pressure-induced amorphization of PdTeI.
2211.10294v1
2023-02-21
Electron transport and scattering mechanisms in ferromagnetic monolayer Fe$_3$GeTe$_2$
We study intrinsic charge-carrier scattering mechanisms and determine their contribution to the transport properties of the two-dimensional ferromagnet Fe$_3$GeTe$_2$. We use state-of-the-art first-principles calculations combined with the model approaches to elucidate the role of the electron-phonon and electron-magnon interactions in the electronic transport. Our findings show that the charge carrier scattering in Fe$_3$GeTe$_2$ is dominated by the electron-phonon interaction, while the role of magnetic excitations is marginal. At the same time, the magnetic ordering is shown to effect essentially on the electron-phonon coupling and its temperature dependence. This leads to a sublinear temperature dependence of the electrical resistivity near the Curie temperature, which is in line with experimental observations. The room temperature resistivity is estimated to be $\sim$35 $\mu \Omega \cdot$cm which may be considered as an intrinsic limit for monolayer Fe$_3$GeTe$_2$.
2302.10974v1
2023-03-20
Thermal decomposition of the Kitaev material $α$-RuCl$_3$ and its influence on low-temperature behavior
We explore the effect of heat treatment in argon atmosphere under various temperatures up to $500^\circ$C on single crystals of $\alpha$-RuCl$_3$ by study of the mass loss, microprobe energy dispersive x-ray spectroscopy, powder x-ray diffraction, electrical resistance as well as low-temperature magnetic susceptibility and specific heat. Clear signatures of dechlorination and oxidation of Ru appear for annealing temperatures beyond $300^\circ$C. Analysis of the specific heat below 2~K reveals a RuO$_2$ mass fraction of order $1\%$ for pristine $\alpha$-RuCl$_3$ which increases up to $20\%$ after thermal annealing, fully consistent with mass-loss analysis. The small RuO$_2$ inclusions drastically reduce the global electrical resistance and may thus significantly affect low-temperature thermal transport and Hall effect.
2303.11308v1
2023-09-08
Re-entrance of resistivity due to the interplay of superconductivity and magnetism in $\ce{Eu_{0.73}Ca_{0.27}(Fe_{0.87}Co_{0.13})2As2}$
By simultaneous Co and Ca-doping we were able to obtain an $\ce{EuFe2As2}$-based compound with superconductivity appearing above the antiferromagnetic order of $\ce{Eu^{2+}}$ magnetic moments. However, as soon as the antiferromagnetic order appears a re-entrance behavior is observed \textemdash{} instead of zero resistivity and diamagnetic signal down to the temperature of \unit[2]{K}. By investigating magnetization, ac susceptibility and electrical transport properties of $\ce{Eu_{0.73}Ca_{0.27}(Fe_{0.87}Co_{0.13})2As2}$ and comparing them to previously studied M\"ossbauer effect and neutron scattering measurements of this and similar compounds an explanation of such behavior is proposed.
2309.04308v2
2023-10-02
Crystallographic-dependent bilinear magnetoelectric resistance in a thin WTe$_2$ layer
The recently reported Bilinear Magnetoeletric Resistance (BMR) in novel materials with rich spin textures, such as bismuth selenide (Bi$_2$Se$_3$) and tungsten ditelluride (WTe$_2$), opens new possibilities for probing the spin textures via magneto-transport measurements. By its nature, the BMR effect is directly linked to the crystal symmetry of the materials and its spin texture. Therefore, understanding the crystallographic dependency of the effect is crucial. Here we report the observation of crystallographic-dependent BMR in thin WTe$_2$ layers and explore how it is linked to its spin textures. The linear response measured in first harmonic signals and the BMR measured in second harmonic signals are both studied under a wide range of magnitudes and directions of magnetic field, applied current and at different temperatures. We discover a three-fold symmetry contribution of the BMR when current is applied along the a-axis of the WTe$_2$ thin layer at 10 K, which is absent for when current is applied along the b-axis.
2310.01058v1
2023-11-23
Helicoidal Transformation Method for Finite Element Models of Twisted Superconductors
This paper deals with the modelling of superconducting and resistive wires with a helicoidal symmetry, subjected to an external field and a transport current. Helicoidal structures are three-dimensional, and therefore yield computationally intensive simulations in a Cartesian coordinate system. We show in this paper that by working instead with a helicoidal system of coordinates, the problem to solve can be made two-dimensional, drastically reducing the computational cost. We first introduce the state-of-the-art approach and apply it on the h-phi-formulation with helicoidally symmetric boundary conditions (e.g., axial external magnetic field, with or without transport current), with an emphasis on the function space discretization. Then, we extend the approach to general boundary conditions (e.g., transverse external magnetic field) and present numerical results with linear materials. In particular, we discuss the frequency-dependent losses in composite wires made of superconducting filaments embedded in a resistive matrix. Finally, we provide outlook to the application of the generalized model with nonlinear materials.
2311.13919v2
2024-03-28
Single-Crystal Growth and Characterization of Cuprate Superconductor (Hg,Re)Ba$_2$Ca$_2$Cu$_3$O$_{8+δ}$
We grew (Hg,Re)Ba$_2$Ca$_2$Cu$_3$O$_{8+\delta}$ ((Hg,Re)1223) single crystals with good reproducibility via the single-step flux method using monoxides as raw materials. A double-sealing method using a thick-walled quartz tube and a stainless-steel container was adopted for explosion protection. The maximum crystal size was approximately 1 mm x 1 mm in the ab plane and 0.04 mm in thickness. The crystal was square-shaped, reflecting the tetragonal crystal structure of (Hg,Re)1223. Magnetic susceptibility measurements indicated a critical temperature of 130 K. The in-plane resistivity exhibited a linear temperature dependence, indicating that the sample was close to optimal doping level. The out-of-plane resistivity was also measured, and the anisotropy parameter was 250-650 at 300 K.
2403.19182v1
2024-05-01
Tunable viscous layers in Corbino geometry using density junctions
In sufficiently clean materials where electron-electron interactions are strong compared to momentum-relaxing scattering processes, electron transport resembles the flow of a viscous fluid. We study hydrodynamic electron transport across density interfaces (n-n junctions) in a 2DEG in the Corbino geometry. From numerical simulations in COMSOL using realistic parameters, we show that we can produce tunable viscous layers at the density interface by varying the density ratio of charge carriers. We quantitatively explain this observation with simple analytic expressions together with boundary conditions at the interface. We also show signatures of these viscous layers in the magnetoresistance. Breaking down viscous and ohmic contributions, we find that when outer radial region of the Corbino has higher charge density compared to the inner region, the viscous layers at the interface serve to suppress the magneto-resistance produced by momentum-relaxing scattering. Conversely, the magneto-resistance is enhanced when the inner region has higher density than the outer. Our results add to the repertoire of techniques for engineering viscous electron flows, which hold a promise for applications in future electronic devices.
2405.00381v1
2003-06-06
Collective transport and optical absorption near the stripe criticality
Within the stripe quantum critical point scenario for high $T_c$ superconductors, we point out the possible direct contribution of charge collective fluctuations to the optical absorption and to the d.c. resistivity.
0306176v1
2010-08-09
Planes, Chains, and Orbits: Quantum Oscillations and High Magnetic Field Heat Capacity in Underdoped YBCO
The underlying physics of the magnetic-field-induced resistive state in high temperature cuprate superconductors remains a mystery. One interpretation is that the application of magnetic field destroys the d-wave superconducting gap to uncover a Fermi surface that behaves like a conventional (i.e.Fermi Liquid) metal (1). Another view is that an applied magnetic field destroys long range superconducting phase coherence, but the superconducting gap amplitude survives (2, 3). By measuring the specific heat of ultra-clean YBa2Cu3O6.56 (YBCO 6.56), we obtain a measure of the quasi-particle density of states from the superconducting state well into the magnetic-field-induced resistive state. We have found that at very high magnetic fields the specific heat exhibits both the conventional temperature dependence and quantum oscillations expected for a Fermi Liquid. On the other hand, the magnetic field dependence of the quasi-particle density of states follows a \sqrt{H} behavior that persists right through the zero-resistance transition, evidencing the fully developed d-wave superconducting gap over the entire magnetic field range measured. The coexistence of these two phenomena pose a rigorous thermodynamic constraint on theories of high-magnetic-field resistive state in the cuprates.
1008.1568v1
2011-02-09
Heavy Long-lived Mossbauer State of Niobium
A heavy niobium state showing 1/3 residual resistance is discovered below the superconducting transition temperature. This niobium sample contains high-density long-lived Mossbauer excitation.
1102.1766v2
2015-12-21
Kondo effect in CeX$_{c}$ (X$_{c}$=S, Se, Te) studied by electrical resistivity under high pressure
We have measured the electrical resistivity of cerium monochalcogenices, CeS, CeSe, and CeTe, under high pressures up to 8 GPa. Pressure dependences of the antiferromagnetic ordering temperature $T_{N}$, crystal field splitting, and the $\ln T$ anomaly of the Kondo effect have been studied to cover the whole region from the magnetic ordering regime at low pressure to the Fermi liquid regime at high pressure. $T_{N}$ initially increases with increasing pressure, and starts to decrease at high pressure as expected from the Doniach's diagram. Simultaneously, the $\ln T$ behavior in the resistivity is enhanced, indicating the enhancement of the Kondo effect by pressure. It is also characteristic in CeX$_{c}$ that the crystal field splitting rapidly decreases at a common rate of $-12.2$ K/GPa. This leads to the increase in the degeneracy of the $f$ state and further enhancement of the Kondo effect. It is shown that the pressure dependent degeneracy of the $f$ state is a key factor to understand the pressure dependence of $T_{N}$, Kondo effect, magnetoresistance, and the peak structure in the temperature dependence of resistivity.
1512.06530v1
2019-10-01
High transparency Bi2Se3 topological insulator nanoribbon Josephson junctions with low resistive noise properties
Bi$_2$Se$_3$ nanoribbons, grown by catalyst-free Physical Vapour Deposition, have been used to fabricate high quality Josephson junctions with Al superconducting electrodes. The conductance spectra (dI/dV) of the junctions show clear dip-peak structures characteristic of multiple Andreev reflections. The temperature dependence of the dip-peak features reveals a highly transparent Al/Bi$_2$Se$_3$ topological insulator nanoribbon interface and Josephson junction barrier. This is supported by the high values of the Bi$_2$Se$_3$ induced gap and of I$_c$R$_n$ (I$_c$ critical current, R$_n$ normal resistance of the junction) product both of the order of 160 $\mu$eV, a value close to the Al gap. The devices present an extremely low relative resistance noise below 1$\times$10$^{-12}$ $\mu$m$^2$/Hz comparable to the best Al tunnel junctions, which indicates a high stability in the transmission coefficients of transport channels. The ideal Al/Bi$_2$Se$_3$ interface properties, perfect transparency for Cooper pair transport in conjunction with low resistive noise make these junctions a suitable platform for further studies of the induced topological superconductivity and Majorana bound states physics.
1910.00280v2
2017-04-28
Electric Field Effect in Multilayer Cr2Ge2Te6: a Ferromagnetic Two-Dimensional Material
The emergence of two-dimensional (2D) materials has attracted a great deal of attention due to their fascinating physical properties and potential applications for future nanoelectronic devices. Since the first isolation of graphene, a Dirac material, a large family of new functional 2D materials have been discovered and characterized, including insulating 2D boron nitride, semiconducting 2D transition metal dichalcogenides and black phosphorus, and superconducting 2D bismuth strontium calcium copper oxide, molybdenum disulphide and niobium selenide, etc. Here, we report the identification of ferromagnetic thin flakes of Cr2Ge2Te6 (CGT) with thickness down to a few nanometers, which provides a very important piece to the van der Waals structures consisting of various 2D materials. We further demonstrate the giant modulation of the channel resistance of 2D CGT devices via electric field effect. Our results illustrate the gate voltage tunability of 2D CGT and the potential of CGT, a ferromagnetic 2D material, as a new functional quantum material for applications in future nanoelectronics and spintronics.
1704.08862v1
2023-09-26
The p-Laplace "Signature" for Quasilinear Inverse Problems with Large Boundary Data
This paper is inspired by an imaging problem encountered in the framework of Electrical Resistance Tomography involving two different materials, one or both of which are nonlinear. Tomography with nonlinear materials is in the early stages of developments, although breakthroughs are expected in the not-too-distant future. We consider nonlinear constitutive relationships which, at a given point in the space, present a behaviour for large arguments that is described by monomials of order p and q. The original contribution this work makes is that the nonlinear problem can be approximated by a weighted p-Laplace problem. From the perspective of tomography, this is a significant result because it highlights the central role played by the $p-$Laplacian in inverse problems with nonlinear materials. Moreover, when p=2, this provides a powerful bridge to bring all the imaging methods and algorithms developed for linear materials into the arena of problems with nonlinear materials. The main result of this work is that for "large" Dirichlet data in the presence of two materials of different order (i) one material can be replaced by either a perfect electric conductor or a perfect electric insulator and (ii) the other material can be replaced by a material giving rise to a weighted p-Laplace problem.
2309.15206v1
2024-04-23
An Accessible Instrument for Measuring Soft Material Mechanical Properties
Soft material research has seen significant growth in recent years, with emerging applications in robotics, electronics, and healthcare diagnostics where understanding material mechanical response is crucial for precision design. Traditional methods for measuring nonlinear mechanical properties of soft materials require specially sized samples that are extracted from their natural environment to be mounted on the testing instrument. This has been shown to compromise data accuracy and precision in various soft and biological materials. To overcome this, the Volume Controlled Cavity Expansion (VCCE) method was developed. This technique tests soft materials by controlling the formation rate of a liquid cavity inside the materials at the tip of an injection needle, and simultaneously measuring the resisting pressure which describes the material response. Despite VCCE's early successes, expansion of its application beyond academia has been hindered by cost, size, and expertise. In response to this, the first portable, bench-top instrument utilizing VCCE is presented here. This device, built with affordable, readily available components and open-source software, streamlines VCCE experimentation without sacrificing performance or precision. It is especially suitable for space-limited settings and designed for use by non-experts, promoting widespread adoption. The instrument's efficacy was demonstrated through testing Polydimethylsiloxane (PDMS) samples of varying stiffness. This study not only validates instrument performance, but also sets the stage for further advancements and broader applications in soft material testing. All data, along with acquisition, control, and post-processing scripts, are made available on GitHub.
2404.15036v1
2018-04-04
High-Performance Flexible Magnetic Tunnel Junctions for Smart Miniaturized Instruments
Flexible electronics is an emerging field in many applications ranging from in vivo biomedical devices to wearable smart systems. The capability of conforming to curved surfaces opens the door to add electronic components to miniaturized instruments, where size and weight are critical parameters. Given their prevalence on the sensors market, flexible magnetic sensors play a major role in this progress. For many high-performance applications, magnetic tunnel junctions (MTJs) have become the first choice, due to their high sensitivity, low power consumption etc. MTJs are also promising candidates for non-volatile next-generation data storage media and, hence, could become central components of wearable electronic devices. In this work, a generic low-cost regenerative batch fabrication process is utilized to transform rigid MTJs on a 500 {\mu}m silicon wafer substrate into 5 {\mu}m thin, mechanically flexible silicon devices, and ensuring optimal utilization of the whole substrate. This method maintains the outstanding magnetic properties, which are only obtained by deposition of the MTJ on smooth high-quality silicon wafers. The flexible MTJs are highly reliable and resistive to mechanical stress. Bending of the MTJ stacks with a diameter as small as 500 {\mu}m is possible without compromising their performance and an endurance of over 1000 cycles without fatigue has been demonstrated. The flexible MTJs were mounted onto the tip of a cardiac catheter with 2 mm in diameter without compromising their performance. This enables the detection of magnetic fields and the angle which they are applied at with a high sensitivity of 4.93 %/Oe and a low power consumption of 0.15 {\mu}W, while adding only 8 {\mu}g and 15 {\mu}m to the weight and diameter of the catheter, respectively.
1804.01298v1
2017-01-30
High quality factor manganese-doped aluminum lumped-element kinetic inductance detectors sensitive to frequencies below 100 GHz
Aluminum lumped-element kinetic inductance detectors (LEKIDs) sensitive to millimeter-wave photons have been shown to exhibit high quality factors, making them highly sensitive and multiplexable. The superconducting gap of aluminum limits aluminum LEKIDs to photon frequencies above 100 GHz. Manganese-doped aluminum (Al-Mn) has a tunable critical temperature and could therefore be an attractive material for LEKIDs sensitive to frequencies below 100 GHz if the internal quality factor remains sufficiently high when manganese is added to the film. To investigate, we measured some of the key properties of Al-Mn LEKIDs. A prototype eight-element LEKID array was fabricated using a 40 nm thick film of Al-Mn deposited on a 500 {\mu}m thick high-resistivity, float-zone silicon substrate. The manganese content was 900 ppm, the measured $T_c = 694\pm1$ mK, and the resonance frequencies were near 150 MHz. Using measurements of the forward scattering parameter $S_{21}$ at various bath temperatures between 65 and 250 mK, we determined that the Al-Mn LEKIDs we fabricated have internal quality factors greater than $2 \times 10^5$, which is high enough for millimeter-wave astrophysical observations. In the dark conditions under which these devices were measured, the fractional frequency noise spectrum shows a shallow slope that depends on bath temperature and probe tone amplitude, which could be two-level system noise. The anticipated white photon noise should dominate this level of low-frequency noise when the detectors are illuminated with millimeter-waves in future measurements. The LEKIDs responded to light pulses from a 1550 nm light-emitting diode, and we used these light pulses to determine that the quasiparticle lifetime is 60 {\mu}s.
1701.08461v2
1997-08-21
Charge Dynamics from Copper Oxide Materials
The charge dynamics of the copper oxide materials in the underdoped and optimal doped regimes is studied within the framework of the fermion-spin theory. The conductivity spectrum shows the non-Drude behavior at low energies and unusual midinfrared peak, and the resistivity exhibits a linear behavior in the temperature, which are consistent with experiments and numerical simulations.
9708165v2
2000-07-06
Scaling of Crack Surfaces and Implications on Fracture Mechanics
The scaling laws describing the roughness development of crack surfaces are incorporated into the Griffith criterion. We show that, in the case of a Family-Vicsek scaling, the energy balance leads to a purely elastic brittle behavior. On the contrary, it appears that an anomalous scaling reflects a R-curve behavior associated to a size effect of the critical resistance to crack growth in agreement with the fracture process of heterogeneous brittle materials exhibiting a microcracking damage.
0007100v1
2001-01-17
Negative Magnetoresistance Produced by Hall Fluctuations in a Ferromagnetic Domain Structure
We present a model for a negative magnetoresistance (MR) that would develop in a material with many ferromagnetic domains even if the individual domains have no magnetoresistance and even if there is no boundary resistance. The negative MR is due to a classical current-distortion effect arising from spatial variations in the Hall conductivity, combined with a change in domain structure due to an applied magnetic field. The negative MR can exceed 1000% if the product of the carrier relaxation time and the internal magnetic field due to spontaneous magnetization is sufficiently large.
0101268v2
2001-03-06
Rheology of a confined granular material
We study the rheology of a granular material slowly driven in a confined geometry. The motion is characterized by a steady sliding with a resistance force increasing with the driving velocity and the surrounding relative humidity. For lower driving velocities a transition to stick-slip motion occurs, exhibiting a blocking enhancement whith decreasing velocity. We propose a model to explain this behavior pointing out the leading role of friction properties between the grains and the container's boundary.
0103143v1
2001-11-07
Crumpling a Thin Sheet
Crumpled sheets have a surprisingly large resistance to further compression. We have studied the crumpling of thin sheets of Mylar under different loading conditions. When placed under a fixed compressive force, the size of a crumpled material decreases logarithmically in time for periods up to three weeks. We also find hysteretic behavior when measuring the compression as a function of applied force. By using a pre-treating protocol, we control this hysteresis and find reproducible scaling behavior for the size of the crumpled material as a function of the applied force.
0111095v1