dataset_id
large_stringclasses
414 values
reaction_id
large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
reactant_smiles
large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-f7c3fa07821a4acd950e43369bfa1625
COC(=O)c1cccc(NCc2cccnc2)c1C(=O)OC>>O=C(O)c1cccc(NCc2cccnc2)c1C(=O)O
COC(C=1C(C(=O)OC)=C(C=CC1)NCC=1C=NC=CC1)=O.COCCNC1=C(C(C(=O)O)=CC=C1)C(=O)O.Cl>>N1=CC(=CC=C1)CNC1=C(C(C(=O)O)=CC=C1)C(=O)O
C[O:3][C:2](=[O:1])[c:4]1[cH:5][cH:6][cH:7][c:8]([NH:9][CH2:10][c:11]2[cH:12][cH:13][cH:14][n:15][cH:16]2)[c:17]1[C:18](=[O:19])[O:20]C>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][cH:7][c:8]([NH:9][CH2:10][c:11]2[cH:12][cH:13][cH:14][n:15][cH:16]2)[c:17]1[C:18](=[O:19])[OH:20]
COC(=O)c1cccc(NCc2cccnc2)c1C(=O)OC
O=C(O)c1cccc(NCc2cccnc2)c1C(=O)O
null
null
null
Deprotection
OtherReaction
6e62db7aac546f574bcfb83067ba8906c30fcbfedfc37aa16b5eaad33833f45a
ed5fed81ba501ef41c88831ec6b9463b899bfdd0815c4145ae51c79addb226d0
c1ccc(NCc2cccnc2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]:[c:5]-[C:6](=[O;D1;H0:7])-[OH;D1;+0:8]
null
[]
null
null
null
null
3-[(Pyridin-3-ylmethyl)-amino]-phthalic acid dimethyl ester (0.91 g, 3.03 mmol) was treated in the same manner as described above for the synthesis of 3-(2-methoxy-ethylamino)-phthalic acid except the pH of crude reaction mixture was adjusted to 2–3 by dropwise addition of concentrated HCl. The solvent was then evapora...
10.6084/m9.figshare.5104873.v1
null
Ester.Ester
Carboxylic acid.Carboxylic acid
null
null
c1ccccc1.c1ccncc1
Other
null
null
null
COC(=O)c1cccc(NCc2cccnc2)c1C(=O)OC>>O=C(O)c1cccc(NCc2cccnc2)c1C(=O)O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-80159be2392144d09e216792dc61590b
COCCNc1cccc2c1C(=O)N(C1CCC(=O)NC1=O)C2=O.O=C(O)c1cccc(NCc2cccnc2)c1C(=O)O>>O=C1CCC(N2C(=O)c3cccc(NCc4cccnc4)c3C2=O)C(=O)N1
N1=CC(=CC=C1)CNC1=C(C(C(=O)O)=CC=C1)C(=O)O.O=C1NC(CCC1N1C(C2=CC=CC(=C2C1=O)NCCOC)=O)=O>>O=C1NC(CCC1N1C(C2=CC=CC(=C2C1=O)NCC=1C=NC=CC1)=O)=O
COCCNc1cccc2c1C(=O)[N:6]([CH:5]1[CH2:4][CH2:3][C:2](=[O:1])[NH:27][C:25]1=[O:26])C2=O.O[C:7](=[O:8])[c:9]1[cH:10][cH:11][cH:12][c:13]([NH:14][CH2:15][c:16]2[cH:17][cH:18][cH:19][n:20][cH:21]2)[c:22]1[C:23](O)=[O:24]>>[O:1]=[C:2]1[CH2:3][CH2:4][CH:5]([N:6]2[C:7](=[O:8])[c:9]3[cH:10][cH:11][cH:12][c:13]([NH:14][CH2:15][c...
COCCNc1cccc2c1C(=O)N(C1CCC(=O)NC1=O)C2=O.O=C(O)c1cccc(NCc2cccnc2)c1C(=O)O
O=C1CCC(N2C(=O)c3cccc(NCc4cccnc4)c3C2=O)C(=O)N1
null
null
CO.C(C)(=O)OCC
Acylation
OtherReaction
5b97b2716363c7d076f525a81453119f9bd234e3df60a591fce8a07715532192
b34812891aa4b14ae9732f1e94ebf3683240312475d27c2db2c5e5699f26030f
O=C1CCC(N2C(=O)c3cccc(NCc4cccnc4)c3C2=O)C(=O)N1
C-O-C-C-N-c1:c:c:c:c2:c:1-C(=O)-[N;H0;D3;+0:1](-[C:2](-[C:3])-[C:4](=[O;D1;H0:5])-[#7:6]-[C:7]=[O;D1;H0:8])-C-2=O.O-[C;H0;D3;+0:9](=[O;D1;H0:10])-[c:11](:[c:12]):[c:13](-[C;H0;D3;+0:14](-O)=[O;D1;H0:15]):[c:16]>>[C:3]-[C:2](-[N;H0;D3;+0:1]1-[C;H0;D3;+0:9](=[O;D1;H0:10])-[c:11](:[c:12]):[c:13](:[c:16])-[C;H0;D3;+0:14]-1...
46
[{"value": 46.0, "product": "O=C1NC(CCC1N1C(C2=CC=CC(=C2C1=O)NCC=1C=NC=CC1)=O)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
3-[(Pyridin-3-ylmethyl)-amino]-phthalic acid (3.03 mmol) was treated in the same manner as described above for the synthesis of 2-(2,6-dioxo-piperidin-3-yl)-4-(2-methoxy-ethylamino)-isoindole-1,3-dione. The solid yellow residue was slurried in 50% methanol/ethyl acetate (20 ml) for 18 h to give 0.50 g (46%) of product ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Carboxylic acid.Ether.Substituted dicarboximide.Secondary amine
Substituted dicarboximide
c1ccc2c(c1)C[NH]C2
c1ccc2c(c1)C[NH]C2
C1CCNCC1.c1ccc2c(c1)C[NH]C2.c1ccncc1
HO-
CO.C(C)(=O)OCC
null
null
COCCNc1cccc2c1C(=O)N(C1CCC(=O)NC1=O)C2=O.O=C(O)c1cccc(NCc2cccnc2)c1C(=O)O>CO.C(C)(=O)OCC>O=C1CCC(N2C(=O)c3cccc(NCc4cccnc4)c3C2=O)C(=O)N1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-bfdcbcc015a04d30a1e301c24a11ffe6
CCCCCNc1cccc(C(=O)OC)c1C(=O)OC.O=Cc1ccc(C(=O)O)o1>>COC(=O)c1cccc(NCc2ccc(C(=O)O)o2)c1C(=O)OC
C(=O)C1=CC=C(O1)C(=O)O.COC(C=1C(C(=O)OC)=C(C=CC1)NCCCCC)=O.C(=O)(O)[O-].[Na+]>>COC(C=1C(C(=O)OC)=C(C=CC1)NCC=1OC(=CC1)C(=O)O)=O
CCCCC[NH:10][c:9]1[cH:8][cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[c:20]1[C:21](=[O:22])[O:23][CH3:24].O=[CH:11][c:12]1[cH:13][cH:14][c:15]([C:16](=[O:17])[OH:18])[o:19]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][cH:8][c:9]([NH:10][CH2:11][c:12]2[cH:13][cH:14][c:15]([C:16](=[O:17])[OH:18])[o:19]2)[c:20]1[C:21](=[O...
CCCCCNc1cccc(C(=O)OC)c1C(=O)OC.O=Cc1ccc(C(=O)O)o1
COC(=O)c1cccc(NCc2ccc(C(=O)O)o2)c1C(=O)OC
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
fc9422fe50863a8e7b22fcc145dd01d982e3de4e7dec633bf5d0e217ba35cfe6
7adcd96acc7986e995a59780d11a29072ec6cdad41c8d7f65df5f25f2d933fc4
c1ccc(NCc2ccco2)cc1
C-C-C-C-C-[NH;D2;+0:1]-[c:2](:[c:3]):[c:4]-[C:5](-[#8:6])=[O;D1;H0:7].O=[CH;D2;+0:8]-[c:9](:[c:10]):[#8;a:11]:[c:12]-[C:13](=[O;D1;H0:14])-[O;D1;H1:15]>>[#8:6]-[C:5](=[O;D1;H0:7])-[c:4]:[c:2](-[NH;D2;+0:1]-[CH2;D2;+0:8]-[c:9](:[c:10]):[#8;a:11]:[c:12]-[C:13](=[O;D1;H0:14])-[O;D1;H1:15]):[c:3]
null
[]
null
null
null
null
5-Formyl-furan-2-carboxylic acid (1 g, 7.14 mmol) was treated in the same manner as described above for the synthesis of 3-pentylamino-phthalic acid dimethyl ester except the combined aqueous NaHCO3 extracts were washed with methylene chloride (1×70 ml) and the pH adjusted to 2–3 by dropwise addition of concentrated HC...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Secondary amine
Secondary amine
null
null
c1ccccc1.c1ccoc1
HO-
null
null
null
CCCCCNc1cccc(C(=O)OC)c1C(=O)OC.O=Cc1ccc(C(=O)O)o1>>COC(=O)c1cccc(NCc2ccc(C(=O)O)o2)c1C(=O)OC
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-a080fa42b94c4d4aa5467f846ef27407
COC(=O)c1cccc(NCc2ccc(C(=O)O)o2)c1C(=O)OC>>O=C(O)c1ccc(CNc2cccc(C(=O)O)c2C(=O)O)o1
COC(C=1C(C(=O)OC)=C(C=CC1)NCC=1OC(=CC1)C(=O)O)=O.COCCNC1=C(C(C(=O)O)=CC=C1)C(=O)O>>C(=O)(O)C1=CC=C(O1)CNC1=C(C(C(=O)O)=CC=C1)C(=O)O
C[O:17][C:15]([c:14]1[cH:13][cH:12][cH:11][c:10]([NH:9][CH2:8][c:7]2[cH:6][cH:5][c:4]([C:2](=[O:1])[OH:3])[o:22]2)[c:18]1[C:19](=[O:20])[O:21]C)=[O:16]>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][c:7]([CH2:8][NH:9][c:10]2[cH:11][cH:12][cH:13][c:14]([C:15](=[O:16])[OH:17])[c:18]2[C:19](=[O:20])[OH:21])[o:22]1
COC(=O)c1cccc(NCc2ccc(C(=O)O)o2)c1C(=O)OC
O=C(O)c1ccc(CNc2cccc(C(=O)O)c2C(=O)O)o1
null
null
null
Deprotection
OtherReaction
6e62db7aac546f574bcfb83067ba8906c30fcbfedfc37aa16b5eaad33833f45a
ed5fed81ba501ef41c88831ec6b9463b899bfdd0815c4145ae51c79addb226d0
c1ccc(NCc2ccco2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]:[c:5]-[C:6](=[O;D1;H0:7])-[OH;D1;+0:8]
null
[]
null
null
null
null
3-[(5-Carboxy-furan-2-ylmethyl)-amino]-phthalic acid dimethyl ester (0.90 g, 2.70 mmol) was treated in the same manner as described above for the synthesis of 3-(2-methoxy-ethylamino)-phthalic acid. The product of the reaction, which contained a mixture of diacid and monomethyl esters, was used without further purifica...
10.6084/m9.figshare.5104873.v1
null
Ester.Ester
Carboxylic acid.Carboxylic acid
null
null
c1ccoc1.c1ccccc1
Other
null
null
null
COC(=O)c1cccc(NCc2ccc(C(=O)O)o2)c1C(=O)OC>>O=C(O)c1ccc(CNc2cccc(C(=O)O)c2C(=O)O)o1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-b56ed8791a944129a68e40b13317ed46
CCCCCNc1cccc(C(=O)OC)c1C(=O)OC.Cc1cc(C=O)oc1C>>COC(=O)c1cccc(NCc2cc(C)c(C)o2)c1C(=O)OC
CC=1C=C(OC1C)C=O.COC(C=1C(C(=O)OC)=C(C=CC1)NCCCCC)=O>>COC(C=1C(C(=O)OC)=C(C=CC1)NCC=1OC(=C(C1)C)C)=O
CCCCC[NH:10][c:9]1[cH:8][cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[c:19]1[C:20](=[O:21])[O:22][CH3:23].O=[CH:11][c:12]1[cH:13][c:14]([CH3:15])[c:16]([CH3:17])[o:18]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][cH:8][c:9]([NH:10][CH2:11][c:12]2[cH:13][c:14]([CH3:15])[c:16]([CH3:17])[o:18]2)[c:19]1[C:20](=[O:21])[O:22...
CCCCCNc1cccc(C(=O)OC)c1C(=O)OC.Cc1cc(C=O)oc1C
COC(=O)c1cccc(NCc2cc(C)c(C)o2)c1C(=O)OC
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
fc9422fe50863a8e7b22fcc145dd01d982e3de4e7dec633bf5d0e217ba35cfe6
7adcd96acc7986e995a59780d11a29072ec6cdad41c8d7f65df5f25f2d933fc4
c1ccc(NCc2ccco2)cc1
C-C-C-C-C-[NH;D2;+0:1]-[c:2](:[c:3]):[c:4]-[C:5](-[#8:6])=[O;D1;H0:7].O=[CH;D2;+0:8]-[c:9](:[c:10]):[#8;a:11]:[c:12]>>[#8:6]-[C:5](=[O;D1;H0:7])-[c:4]:[c:2](-[NH;D2;+0:1]-[CH2;D2;+0:8]-[c:9](:[c:10]):[#8;a:11]:[c:12]):[c:3]
75
[{"value": 75.0, "product": "COC(C=1C(C(=O)OC)=C(C=CC1)NCC=1OC(=C(C1)C)C)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
4,5-Dimethyl-furan-2-carbaldehyde (0.98 ml, 8 mmol) was treated in the same manner as described above for the synthesis of 3-pentylamino-phthalic acid dimethyl ester. The residue (oil) was purified by chromatography (SiO2, 10% ethyl acetate/hexanes) to give 0.95 g (75%) of product as a yellow oil: 1H NMR (CDCl3) δ 7.32...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Secondary amine
Secondary amine
null
null
c1ccccc1.c1ccoc1
HO-
null
null
null
CCCCCNc1cccc(C(=O)OC)c1C(=O)OC.Cc1cc(C=O)oc1C>>COC(=O)c1cccc(NCc2cc(C)c(C)o2)c1C(=O)OC
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-cfa84e91e6c94d06b8e67c3313c14f77
COC(=O)c1cccc(NCc2cc(C)c(C)o2)c1C(=O)OC>>Cc1cc(CNc2cccc(C(=O)O)c2C(=O)O)oc1C
COC(C=1C(C(=O)OC)=C(C=CC1)NCC=1OC(=C(C1)C)C)=O.COCCNC1=C(C(C(=O)O)=CC=C1)C(=O)O>>CC=1C=C(OC1C)CNC1=C(C(C(=O)O)=CC=C1)C(=O)O
C[O:14][C:12]([c:11]1[cH:10][cH:9][cH:8][c:7]([NH:6][CH2:5][c:4]2[cH:3][c:2]([CH3:1])[c:20]([CH3:21])[o:19]2)[c:15]1[C:16](=[O:17])[O:18]C)=[O:13]>>[CH3:1][c:2]1[cH:3][c:4]([CH2:5][NH:6][c:7]2[cH:8][cH:9][cH:10][c:11]([C:12](=[O:13])[OH:14])[c:15]2[C:16](=[O:17])[OH:18])[o:19][c:20]1[CH3:21]
COC(=O)c1cccc(NCc2cc(C)c(C)o2)c1C(=O)OC
Cc1cc(CNc2cccc(C(=O)O)c2C(=O)O)oc1C
null
null
null
Deprotection
OtherReaction
6e62db7aac546f574bcfb83067ba8906c30fcbfedfc37aa16b5eaad33833f45a
ed5fed81ba501ef41c88831ec6b9463b899bfdd0815c4145ae51c79addb226d0
c1ccc(NCc2ccco2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]:[c:5]-[C:6](=[O;D1;H0:7])-[OH;D1;+0:8]
null
[]
null
null
null
null
3-[(4,5-Dimethyl-furan-2-ylmethyl)-amino]-phthalic acid dimethyl ester (0.95 g, 3 mmol) was treated in the same manner as described above for the synthesis of 3-(2-methoxy-ethylamino)-phthalic acid. The product of the reaction, which contained a mixture of diacid and monomethyl esters, was used without further purifica...
10.6084/m9.figshare.5104873.v1
null
Ester.Ester
Carboxylic acid.Carboxylic acid
null
null
c1ccoc1.c1ccccc1
Other
null
null
null
COC(=O)c1cccc(NCc2cc(C)c(C)o2)c1C(=O)OC>>Cc1cc(CNc2cccc(C(=O)O)c2C(=O)O)oc1C
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-9c6b1c3d12724d2c8737b896e74c04dc
COCCNc1cccc2c1C(=O)N(C1CCC(=O)NC1=O)C2=O.Cc1cc(CNc2cccc(C(=O)O)c2C(=O)O)oc1C>>Cc1cc(CNc2cccc3c2C(=O)N(C2CCC(=O)NC2=O)C3=O)oc1C
CC=1C=C(OC1C)CNC1=C(C(C(=O)O)=CC=C1)C(=O)O.O=C1NC(CCC1N1C(C2=CC=CC(=C2C1=O)NCCOC)=O)=O>>CC=1C=C(OC1C)CNC1=C2C(N(C(C2=CC=C1)=O)C1C(NC(CC1)=O)=O)=O
COCCNc1cccc2c1[C:13](=[O:14])[N:15]([CH:16]1[CH2:17][CH2:18][C:19](=[O:20])[NH:21][C:22]1=[O:23])[C:24]2=[O:25].O=C(O)[c:11]1[cH:10][cH:9][cH:8][c:7]([NH:6][CH2:5][c:4]2[cH:3][c:2]([CH3:1])[c:27]([CH3:28])[o:26]2)[c:12]1C(=O)O>>[CH3:1][c:2]1[cH:3][c:4]([CH2:5][NH:6][c:7]2[cH:8][cH:9][cH:10][c:11]3[c:12]2[C:13](=[O:14])...
COCCNc1cccc2c1C(=O)N(C1CCC(=O)NC1=O)C2=O.Cc1cc(CNc2cccc(C(=O)O)c2C(=O)O)oc1C
Cc1cc(CNc2cccc3c2C(=O)N(C2CCC(=O)NC2=O)C3=O)oc1C
null
null
null
C-C Coupling
OtherReaction
e01b406c4bd6fd113e0f2e1f0fbdfa1994fad43c14b9a159b5c537e52be3a29d
47dba274a38dfe0abc81230fe8a80653f556b2eb304748f9abffbd031c5d793d
O=C1CCC(N2C(=O)c3cccc(NCc4ccco4)c3C2=O)C(=O)N1
C-O-C-C-N-c1:c:c:c:c2:c:1-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#7:3](-[C:4]-[C:5](=[O;D1;H0:6])-[#7:7])-[C;H0;D3;+0:8]-2=[O;D1;H0:9].O-C(=O)-[c;H0;D3;+0:10]1:[c:11]:[c:12]:[c:13]:[c:14](-[#7:15]):[c;H0;D3;+0:16]:1-C(-O)=O>>[#7:7]-[C:5](=[O;D1;H0:6])-[C:4]-[#7:3]1-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c;H0;D3;+0:16]2:[c:14](-[#7:15]):...
22
[{"value": 22.0, "product": "CC=1C=C(OC1C)CNC1=C2C(N(C(C2=CC=C1)=O)C1C(NC(CC1)=O)=O)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
3-[(4,5-Dimethyl-furan-2-ylmethyl)-amino]-phthalic acid (3 mmol) was treated in the same manner as described above for the synthesis of 2-(2,6-dioxo-piperidin-3-yl)-4-(2-methoxy-ethylamino)-isoindole-1,3-dione. The solid yellow residue was purified by preparative HPLC (Symmetry C18, isocratic, 40% acetonitrile/water) t...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Carboxylic acid.Ether.Substituted dicarboximide.Secondary amine
Substituted dicarboximide
c1ccc2c(c1)C[NH]C2.c1ccccc1
c1ccc2c(c1)C[NH]C2
c1ccoc1.c1ccc2c(c1)C[NH]C2.C1CCNCC1
HO-
null
null
null
COCCNc1cccc2c1C(=O)N(C1CCC(=O)NC1=O)C2=O.Cc1cc(CNc2cccc(C(=O)O)c2C(=O)O)oc1C>>Cc1cc(CNc2cccc3c2C(=O)N(C2CCC(=O)NC2=O)C3=O)oc1C
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-824e5a7e96704e8592397388d933559a
CCCCCNc1cccc(C(=O)OC)c1C(=O)OC.O=Cc1cc2ccccc2o1>>COC(=O)c1cccc(NCc2cc3ccccc3o2)c1C(=O)OC
O1C(=CC2=C1C=CC=C2)C=O.COC(C=1C(C(=O)OC)=C(C=CC1)NCCCCC)=O>>COC(C=1C(C(=O)OC)=C(C=CC1)NCC=1OC2=C(C1)C=CC=C2)=O
CCCCC[NH:10][c:9]1[cH:8][cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[c:21]1[C:22](=[O:23])[O:24][CH3:25].O=[CH:11][c:12]1[cH:13][c:14]2[cH:15][cH:16][cH:17][cH:18][c:19]2[o:20]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][cH:8][c:9]([NH:10][CH2:11][c:12]2[cH:13][c:14]3[cH:15][cH:16][cH:17][cH:18][c:19]3[o:20]2)[c:21]1...
CCCCCNc1cccc(C(=O)OC)c1C(=O)OC.O=Cc1cc2ccccc2o1
COC(=O)c1cccc(NCc2cc3ccccc3o2)c1C(=O)OC
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
fc9422fe50863a8e7b22fcc145dd01d982e3de4e7dec633bf5d0e217ba35cfe6
7adcd96acc7986e995a59780d11a29072ec6cdad41c8d7f65df5f25f2d933fc4
c1ccc(NCc2cc3ccccc3o2)cc1
C-C-C-C-C-[NH;D2;+0:1]-[c:2](:[c:3]):[c:4]-[C:5](-[#8:6])=[O;D1;H0:7].O=[CH;D2;+0:8]-[c:9](:[c:10]):[#8;a:11]:[c:12]>>[#8:6]-[C:5](=[O;D1;H0:7])-[c:4]:[c:2](-[NH;D2;+0:1]-[CH2;D2;+0:8]-[c:9](:[c:10]):[#8;a:11]:[c:12]):[c:3]
83
[{"value": 83.0, "product": "COC(C=1C(C(=O)OC)=C(C=CC1)NCC=1OC2=C(C1)C=CC=C2)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
Benzofuran-2-carbaldehyde (1.17 ml, 8 mmol) was treated in the same manner as described above for the synthesis of 3-pentylamino-phthalic acid dimethyl ester. The residue (oil) was purified by chromatography (SiO2, 50% methylene chloride/hexane) to give 1.12 g (83%) of product as a yellow oil: 1H NMR (CDCl3) δ 7.50–7.4...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Secondary amine
Secondary amine
null
null
c1ccccc1.c1ccc2occc2c1
HO-
null
null
null
CCCCCNc1cccc(C(=O)OC)c1C(=O)OC.O=Cc1cc2ccccc2o1>>COC(=O)c1cccc(NCc2cc3ccccc3o2)c1C(=O)OC
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-5bf4a66bcb92491d9327c32bce841ed3
COC(=O)c1cccc(NCc2cc3ccccc3o2)c1C(=O)OC>>O=C(O)c1cccc(NCc2cc3ccccc3o2)c1C(=O)O
COC(C=1C(C(=O)OC)=C(C=CC1)NCC=1OC2=C(C1)C=CC=C2)=O.COCCNC1=C(C(C(=O)O)=CC=C1)C(=O)O>>O1C(=CC2=C1C=CC=C2)CNC2=C(C(C(=O)O)=CC=C2)C(=O)O
C[O:3][C:2](=[O:1])[c:4]1[cH:5][cH:6][cH:7][c:8]([NH:9][CH2:10][c:11]2[cH:12][c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]3[o:19]2)[c:20]1[C:21](=[O:22])[O:23]C>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][cH:7][c:8]([NH:9][CH2:10][c:11]2[cH:12][c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]3[o:19]2)[c:20]1[C:21](=[O:22])[OH:23]
COC(=O)c1cccc(NCc2cc3ccccc3o2)c1C(=O)OC
O=C(O)c1cccc(NCc2cc3ccccc3o2)c1C(=O)O
null
null
null
Deprotection
OtherReaction
6e62db7aac546f574bcfb83067ba8906c30fcbfedfc37aa16b5eaad33833f45a
ed5fed81ba501ef41c88831ec6b9463b899bfdd0815c4145ae51c79addb226d0
c1ccc(NCc2cc3ccccc3o2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C>>[O;D1;H0:7]=[C:6](-[OH;D1;+0:8])-[c:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
null
[]
null
null
null
null
3-[(Benzofuran-2-ylmethyl)-amino]-phthalic acid dimethyl ester (1.12 g, 3.3 mmol) was treated in the same manner as described above for the synthesis of 3-(2-methoxy-ethylamino)-phthalic acid. The product of the reaction, which contained a mixture of diacid and monomethyl esters, was used without further purification. ...
10.6084/m9.figshare.5104873.v1
null
Ester.Ester
Carboxylic acid.Carboxylic acid
null
null
c1ccccc1.c1ccc2occc2c1
Other
null
null
null
COC(=O)c1cccc(NCc2cc3ccccc3o2)c1C(=O)OC>>O=C(O)c1cccc(NCc2cc3ccccc3o2)c1C(=O)O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-50cf84589f7c499782957520107cf0c1
CC1(N)CCC(=O)NC1=O.O=C(O)c1cccc(NCc2cccc(Cl)c2)c1C(=O)O>>CC1(N2C(=O)c3cccc(NCc4cccc(Cl)c4)c3C2=O)CCC(=O)NC1=O
ClC=1C=C(CNC2=C(C(C(=O)O)=CC=C2)C(=O)O)C=CC1.Cl.NC1(C(NC(CC1)=O)=O)C>>ClC=1C=C(CNC2=C3C(N(C(C3=CC=C2)=O)C2(C(NC(CC2)=O)=O)C)=O)C=CC1
[CH3:1][C:2]1([NH2:3])[CH2:23][CH2:24][C:25](=[O:26])[NH:27][C:28]1=[O:29].O[C:4](=[O:5])[c:6]1[cH:7][cH:8][cH:9][c:10]([NH:11][CH2:12][c:13]2[cH:14][cH:15][cH:16][c:17]([Cl:18])[cH:19]2)[c:20]1[C:21](O)=[O:22]>>[CH3:1][C:2]1([N:3]2[C:4](=[O:5])[c:6]3[cH:7][cH:8][cH:9][c:10]([NH:11][CH2:12][c:13]4[cH:14][cH:15][cH:16][...
CC1(N)CCC(=O)NC1=O.O=C(O)c1cccc(NCc2cccc(Cl)c2)c1C(=O)O
CC1(N2C(=O)c3cccc(NCc4cccc(Cl)c4)c3C2=O)CCC(=O)NC1=O
null
null
N1=CC=CC=C1
Acylation
OtherReaction
03989296fe7fd00d3061010c1aadbbfb4b9eaa9ca91856790fffb1e1bf4b4c50
b7eb222f11e89f2ccff57aab9a5106ae4173f0ba94ac518e1a9f3b22a378531d
O=C1CCC(N2C(=O)c3cccc(NCc4ccccc4)c3C2=O)C(=O)N1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[C;H0;D3;+0:6](-O)=[O;D1;H0:7]):[c:8].[C:9]-[C:10](-[C;D1;H3:11])(-[NH2;D1;+0:12])-[C:13](=[O;D1;H0:14])-[#7:15]-[C:16]=[O;D1;H0:17]>>[C:9]-[C:10](-[C;D1;H3:11])(-[N;H0;D3;+0:12]1-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](:[c:8])-[C;H0;D3;+0:6]-1=[O;D1;H0:7])-[...
41
[{"value": 41.0, "product": "ClC=1C=C(CNC2=C3C(N(C(C3=CC=C2)=O)C2(C(NC(CC2)=O)=O)C)=O)C=CC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 40.7, "product": "ClC=1C=C(CNC2=C3C(N(C(C3=CC=C2)=O)C2(C(NC(CC2)=O)=O)C)=O)C=CC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a stirred solution of 3-(3-Chloro-benzylamino)-phthalic acid (4 mmol) in pyridine (50 ml) was added 3-amino-3-methyl-piperidine-2,6-dione hydrochloride (0.71 g, 4 mmol). The reaction mixture was heated to reflux for 18 h. The solvent was evaporated in vacuo and the residue dissolved in methylene chloride (150 ml). T...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Carboxylic acid.Primary amine
Substituted dicarboximide
null
c1ccc2c(c1)C[NH]C2
c1ccc2c(c1)C[NH]C2.c1ccccc1.C1CCNCC1
HO-
N1=CC=CC=C1
null
null
CC1(N)CCC(=O)NC1=O.O=C(O)c1cccc(NCc2cccc(Cl)c2)c1C(=O)O>N1=CC=CC=C1>CC1(N2C(=O)c3cccc(NCc4cccc(Cl)c4)c3C2=O)CCC(=O)NC1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-1cc65329f18949559358be5e5faca254
Nc1cccc2c1CN(C1CCC(=O)NC1=O)C2=O.O=Cc1cccc(Cl)c1>>O=C1CCC(N2Cc3c(NCc4cccc(Cl)c4)cccc3C2=O)C(=O)N1
C(Cl)Cl.CO.ClC=1C=C(C=O)C=CC1.NC1=C2CN(C(C2=CC=C1)=O)C1C(NC(CC1)=O)=O.C(C)(=O)O[BH-](OC(C)=O)OC(C)=O.[Na+]>>ClC=1C=C(CNC2=C3CN(C(C3=CC=C2)=O)C2C(NC(CC2)=O)=O)C=CC1
[O:1]=[C:2]1[CH2:3][CH2:4][CH:5]([N:6]2[CH2:7][c:8]3[c:9]([NH2:10])[cH:19][cH:20][cH:21][c:22]3[C:23]2=[O:24])[C:25](=[O:26])[NH:27]1.O=[CH:11][c:12]1[cH:13][cH:14][cH:15][c:16]([Cl:17])[cH:18]1>>[O:1]=[C:2]1[CH2:3][CH2:4][CH:5]([N:6]2[CH2:7][c:8]3[c:9]([NH:10][CH2:11][c:12]4[cH:13][cH:14][cH:15][c:16]([Cl:17])[cH:18]4...
Nc1cccc2c1CN(C1CCC(=O)NC1=O)C2=O.O=Cc1cccc(Cl)c1
O=C1CCC(N2Cc3c(NCc4cccc(Cl)c4)cccc3C2=O)C(=O)N1
null
null
C(C)(=O)O.C(Cl)Cl
Heteroatom Alkylation and Arylation
Reductive amination with aldehyde
422be648aea52bce28ccc8fb32ec3178aaa47bbd624f063874619362f075b5f2
7915721a3e395aed85e3c40dc4d725c571a931ac517c6a0da16f2a2b0bb5eac7
O=C1CCC(N2Cc3c(NCc4ccccc4)cccc3C2=O)C(=O)N1
O=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4].[NH2;D1;+0:5]-[c:6](:[c:7]):[c:8]>>[c:3]:[c:2](-[CH2;D2;+0:1]-[NH;D2;+0:5]-[c:6](:[c:7]):[c:8]):[c:4]
31.3
[{"value": 31.0, "product": "ClC=1C=C(CNC2=C3CN(C(C3=CC=C2)=O)C2C(NC(CC2)=O)=O)C=CC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 31.3, "product": "ClC=1C=C(CNC2=C3CN(C(C3=CC=C2)=O)C2C(NC(CC2)=O)=O)C=CC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
3-(4-Amino-1-oxo-1,3-dihydro-isoindol-2-yl)-piperidine-2,6-dione (1.04 g, 4 mmol) was dissolved in acetic acid (7 ml) with heat. The mixture was cooled slightly and methylene chloride (50 ml) was added slowly followed by 3-chlorobenzaldehyde (0.91 ml, 8 mmol) and sodium triacetoxyborohydride (2.54 g, 12 mmol). The reac...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary amine
Secondary amine
null
null
C1CCNCC1.c1ccccc1.c1ccc2c(c1)C[NH]C2
Other
C(C)(=O)O.C(Cl)Cl
null
2
Nc1cccc2c1CN(C1CCC(=O)NC1=O)C2=O.O=Cc1cccc(Cl)c1>C(C)(=O)O.C(Cl)Cl>O=C1CCC(N2Cc3c(NCc4cccc(Cl)c4)cccc3C2=O)C(=O)N1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-285cbc720c8f452cbfe1d2b20c8ade69
NCc1cccc2c1C(=O)N(C1CCC(=O)NC1=O)C2=O.O=C([O-])N(c1ccc([N+](=O)[O-])cc1)C1CCCC1>>O=C1CCC(N2C(=O)c3cccc(CNC(=O)NC4CCCC4)c3C2=O)C(=O)N1
N12CCCCCC2=NCCC1.Cl.NCC1=C2C(N(C(C2=CC=C1)=O)C1C(NC(CC1)=O)=O)=O.[N+](=O)([O-])C1=CC=C(C=C1)N(C([O-])=O)C1CCCC1>>O=C1NC(CCC1N1C(C2=CC=CC(=C2C1=O)CNC(=O)NC1CCCC1)=O)=O
[O:1]=[C:2]1[CH2:3][CH2:4][CH:5]([N:6]2[C:7](=[O:8])[c:9]3[cH:10][cH:11][cH:12][c:13]([CH2:14][NH2:15])[c:24]3[C:25]2=[O:26])[C:27](=[O:28])[NH:29]1.O=[N+]([O-])c1ccc([N:18]([C:16]([O-])=[O:17])[CH:19]2[CH2:20][CH2:21][CH2:22][CH2:23]2)cc1>>[O:1]=[C:2]1[CH2:3][CH2:4][CH:5]([N:6]2[C:7](=[O:8])[c:9]3[cH:10][cH:11][cH:12]...
NCc1cccc2c1C(=O)N(C1CCC(=O)NC1=O)C2=O.O=C([O-])N(c1ccc([N+](=O)[O-])cc1)C1CCCC1
O=C1CCC(N2C(=O)c3cccc(CNC(=O)NC4CCCC4)c3C2=O)C(=O)N1
null
null
C(C)#N
Acylation
OtherReaction
c544444e833963de17b7285ecf254c119edba4524de2ca959e1686976f0aeaf8
75a79f455fef00f73470f8263f7f62d9ceebfd06076631fa20de1d0098d3252f
O=C1CCC(N2C(=O)c3cccc(CNC(=O)NC4CCCC4)c3C2=O)C(=O)N1
O=[N+](-[O-])-c1:c:c:c(-[N;H0;D3;+0:1](-[C:2](-[C:3])-[C:4])-[C;H0;D3;+0:5](-[O-])=[O;D1;H0:6]):c:c:1.[NH2;D1;+0:7]-[C:8]-[c:9]>>[C:3]-[C:2](-[NH;D2;+0:1]-[C;H0;D3;+0:5](=[O;D1;H0:6])-[NH;D2;+0:7]-[C:8]-[c:9])-[C:4]
27.1
[{"value": 27.0, "product": "O=C1NC(CCC1N1C(C2=CC=CC(=C2C1=O)CNC(=O)NC1CCCC1)=O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 27.1, "product": "O=C1NC(CCC1N1C(C2=CC=CC(=C2C1=O)CNC(=O)NC1CCCC1)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
20
MINUTE
1,8-Diazabicyclo[5,4,0]undec-7-ene (0.29 g, 1.9 mmol) was added to a stirred suspension of 4-(aminomethyl)-2-(2,6-dioxo(3-piperidyl))isoindoline-1,3-dione hydrochloride (0.6 g, 1.85 mmol) in acetonitrile (50 mL). After stirring for 20 min, 4-nitrophenyl-N-cyclopentylcarbamate (0.44 g, 1.85 mmol) was added. The mixture ...
10.6084/m9.figshare.5104873.v1
null
Carbamic acid.Nitro group.Primary amine
Urea
c1ccccc1
null
C1CCNCC1.c1ccc2c(c1)C[NH]C2.C1CCCC1
HO-
C(C)#N
null
0.333333
NCc1cccc2c1C(=O)N(C1CCC(=O)NC1=O)C2=O.O=C([O-])N(c1ccc([N+](=O)[O-])cc1)C1CCCC1>C(C)#N>O=C1CCC(N2C(=O)c3cccc(CNC(=O)NC4CCCC4)c3C2=O)C(=O)N1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-14435ce5619b43098a6af1585e7826cd
NCc1cccc2c1C(=O)N(C1CCC(=O)NC1=O)C2=O.O=C(Nc1cccnc1)ON1C(=O)CCC1=O>>O=C1CCC(N2C(=O)c3cccc(CNC(=O)Nc4cccnc4)c3C2=O)C(=O)N1
N12CCCCCC2=NCCC1.Cl.NCC1=C2C(N(C(C2=CC=C1)=O)C1C(NC(CC1)=O)=O)=O.O=C1N(C(CC1)=O)OC(=O)NC=1C=NC=CC1>>O=C1NC(CCC1N1C(C2=CC=CC(=C2C1=O)CNC(=O)NC=1C=NC=CC1)=O)=O
[O:1]=[C:2]1[CH2:3][CH2:4][CH:5]([N:6]2[C:7](=[O:8])[c:9]3[cH:10][cH:11][cH:12][c:13]([CH2:14][NH2:15])[c:25]3[C:26]2=[O:27])[C:28](=[O:29])[NH:30]1.O=C1CCC(=O)N1O[C:16](=[O:17])[NH:18][c:19]1[cH:20][cH:21][cH:22][n:23][cH:24]1>>[O:1]=[C:2]1[CH2:3][CH2:4][CH:5]([N:6]2[C:7](=[O:8])[c:9]3[cH:10][cH:11][cH:12][c:13]([CH2:...
NCc1cccc2c1C(=O)N(C1CCC(=O)NC1=O)C2=O.O=C(Nc1cccnc1)ON1C(=O)CCC1=O
O=C1CCC(N2C(=O)c3cccc(CNC(=O)Nc4cccnc4)c3C2=O)C(=O)N1
null
null
C(C)#N
Acylation
OtherReaction
b72231f0ce68d14b82c0b5dc8e77bb0358ffec1497faa29a27840d8959aefbc2
943dda93229373d8af3aaa08ae8db106d934de8921eb40cdbdad7b33a1554bea
O=C1CCC(N2C(=O)c3cccc(CNC(=O)Nc4cccnc4)c3C2=O)C(=O)N1
O=C1-C-C-C(=O)-N-1-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#7:3]-[c:4]:[c:5]:[#7;a:6].[NH2;D1;+0:7]-[C:8]-[c:9]>>[#7;a:6]:[c:5]:[c:4]-[#7:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:7]-[C:8]-[c:9]
30.5
[{"value": 30.0, "product": "O=C1NC(CCC1N1C(C2=CC=CC(=C2C1=O)CNC(=O)NC=1C=NC=CC1)=O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 30.5, "product": "O=C1NC(CCC1N1C(C2=CC=CC(=C2C1=O)CNC(=O)NC=1C=NC=CC1)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
20
MINUTE
1,8-Diazabicyclo[5,4,0]undec-7-ene (0.29 g, 1.9 mmol) was added to a stirred suspension of 4-(aminomethyl)-2-(2,6-dioxo(3-piperidyl))isoindoline-1,3-dione hydrochloride (0.6 g, 1.85 mmol) in acetonitrile (50 mL). After stirring for 20 min, (2,5-dioxopyrrolidinyloxy)-N-(3-pyridyl)carboxamide (0.44 g, 1.85 mmol) was adde...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Tertiary amide.Tertiary amide.Primary amine
Urea
C1CCNC1
null
C1CCNCC1.c1ccc2c(c1)C[NH]C2.c1ccncc1
HO-
C(C)#N
null
0.333333
NCc1cccc2c1C(=O)N(C1CCC(=O)NC1=O)C2=O.O=C(Nc1cccnc1)ON1C(=O)CCC1=O>C(C)#N>O=C1CCC(N2C(=O)c3cccc(CNC(=O)Nc4cccnc4)c3C2=O)C(=O)N1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-6dfb46c1d0d3403ba8b916c2274dc7e4
O=C1CCC(N2C(=O)c3cccc(CNC(=O)Nc4cccnc4)c3C2=O)C(=O)N1>>O=C1CCC(N2C(=O)c3cccc(CNC(=O)Nc4cccnc4)c3C2=O)C(=O)N1
Cl.CCOCC.O=C1NC(CCC1N1C(C2=CC=CC(=C2C1=O)CNC(=O)NC=1C=NC=CC1)=O)=O>>Cl.O=C1NC(CCC1N1C(C2=CC=CC(=C2C1=O)CNC(=O)NC=1C=NC=CC1)=O)=O
[O:2]=[C:3]1[CH2:4][CH2:5][CH:6]([N:7]2[C:8](=[O:9])[c:10]3[cH:11][cH:12][cH:13][c:14]([CH2:15][NH:16][C:17](=[O:18])[NH:19][c:20]4[cH:21][cH:22][cH:23][n:24][cH:25]4)[c:26]3[C:27]2=[O:28])[C:29](=[O:30])[NH:31]1>>[O:2]=[C:3]1[CH2:4][CH2:5][CH:6]([N:7]2[C:8](=[O:9])[c:10]3[cH:11][cH:12][cH:13][c:14]([CH2:15][NH:16][C:1...
O=C1CCC(N2C(=O)c3cccc(CNC(=O)Nc4cccnc4)c3C2=O)C(=O)N1
O=C1CCC(N2C(=O)c3cccc(CNC(=O)Nc4cccnc4)c3C2=O)C(=O)N1
null
null
CO.C(C)(=O)OCC
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
O=C1CCC(N2C(=O)c3cccc(CNC(=O)Nc4cccnc4)c3C2=O)C(=O)N1
null
null
[]
null
null
2
HOUR
1,8-Diazabicyclo[5,4,0]undec-7-ene (0.29 g, 1.9 mmol) was added to a stirred suspension of 4-(aminomethyl)-2-(2,6-dioxo(3-piperidyl))isoindoline-1,3-dione hydrochloride (0.6 g, 1.85 mmol) in acetonitrile (50 mL). After stirring for 20 min, (2,5-dioxopyrrolidinyloxy)-N-(3-pyridyl)carboxamide (0.44 g, 1.85 mmol) was adde...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
C1CCNCC1.c1ccc2c(c1)C[NH]C2.c1ccncc1
null
CO.C(C)(=O)OCC
null
2
O=C1CCC(N2C(=O)c3cccc(CNC(=O)Nc4cccnc4)c3C2=O)C(=O)N1>CO.C(C)(=O)OCC>O=C1CCC(N2C(=O)c3cccc(CNC(=O)Nc4cccnc4)c3C2=O)C(=O)N1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-7b92f50d6bca4235a268ecf58899edd0
C1CCNCC1.NCc1cccc2c1C(=O)N(C1CCC(=O)NC1=O)C2=O.O=C(OC(Cl)(Cl)Cl)OC(Cl)(Cl)Cl>>O=C1CCC(N2C(=O)c3cccc(CNC(=O)N4CCCCC4)c3C2=O)C(=O)N1
C(C)(C)N(CC)C(C)C.Cl.NCC1=C2C(N(C(C2=CC=C1)=O)C1C(NC(CC1)=O)=O)=O.N1CCCCC1.C(C)(C)N(CC)C(C)C.ClC(Cl)(OC(OC(Cl)(Cl)Cl)=O)Cl>>O=C1NC(CCC1N1C(C2=CC=CC(=C2C1=O)CNC(=O)N1CCCCC1)=O)=O
[NH:18]1[CH2:19][CH2:20][CH2:21][CH2:22][CH2:23]1.[O:1]=[C:2]1[CH2:3][CH2:4][CH:5]([N:6]2[C:7](=[O:8])[c:9]3[cH:10][cH:11][cH:12][c:13]([CH2:14][NH2:15])[c:24]3[C:25]2=[O:26])[C:27](=[O:28])[NH:29]1.ClC(Cl)(Cl)O[C:16](OC(Cl)(Cl)Cl)=[O:17]>>[O:1]=[C:2]1[CH2:3][CH2:4][CH:5]([N:6]2[C:7](=[O:8])[c:9]3[cH:10][cH:11][cH:12][...
C1CCNCC1.NCc1cccc2c1C(=O)N(C1CCC(=O)NC1=O)C2=O.O=C(OC(Cl)(Cl)Cl)OC(Cl)(Cl)Cl
O=C1CCC(N2C(=O)c3cccc(CNC(=O)N4CCCCC4)c3C2=O)C(=O)N1
null
null
C(C)#N
Acylation
OtherReaction
075e010aa242d893511507e9999273f6e4aaf78621d38d5b583bb121b24aa032
a171696b7de78dbbbc9cc830c802d29643daeae80133889bf27fba2e22ed8263
O=C1CCC(N2C(=O)c3cccc(CNC(=O)N4CCCCC4)c3C2=O)C(=O)N1
Cl-C(-Cl)(-Cl)-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-O-C(-Cl)(-Cl)-Cl.[C:3]-[C:4]-[NH;D2;+0:5]-[C:6]-[C:7].[NH2;D1;+0:8]-[C:9]-[c:10]>>[C:3]-[C:4]-[N;H0;D3;+0:5](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:8]-[C:9]-[c:10])-[C:6]-[C:7]
145.3
[{"value": 53.0, "product": "O=C1NC(CCC1N1C(C2=CC=CC(=C2C1=O)CNC(=O)N1CCCCC1)=O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 145.3, "product": "O=C1NC(CCC1N1C(C2=CC=CC(=C2C1=O)CNC(=O)N1CCCCC1)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
20
MINUTE
Diisopropylethylamine (0.88 g, 6.79 mmol) was added to a stirred suspension of 4-(aminomethyl)-2-(2,6-dioxo(3-piperidyl))isoindoline-1,3-dione hydrochloride (1.0 g, 3.09 mmol) in acetonitrile (50 mL). After stirring for 20 min, the mixture was slowly added to a stirred solution of triphosgene (0.34 g, 1.14 mmol) in ace...
10.6084/m9.figshare.5104873.v1
null
Trichloro group.Trichloro group.Carbonic Ester.Primary amine.Secondary amine
Urea
C1CCNCC1
C1CC[NH]CC1
C1CCNCC1.c1ccc2c(c1)C[NH]C2.C1CC[NH]CC1
HCl
C(C)#N
null
0.333333
C1CCNCC1.NCc1cccc2c1C(=O)N(C1CCC(=O)NC1=O)C2=O.O=C(OC(Cl)(Cl)Cl)OC(Cl)(Cl)Cl>C(C)#N>O=C1CCC(N2C(=O)c3cccc(CNC(=O)N4CCCCC4)c3C2=O)C(=O)N1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-515a075d965b456ab2907b2f8edaf345
CI.Cc1c(Br)cccc1C(=O)O>>COC(=O)c1cccc(Br)c1C
BrC=1C(=C(C(=O)O)C=CC1)C.C([O-])(O)=O.[Na+].IC>>BrC=1C(=C(C(=O)OC)C=CC1)C
I[CH3:1].[OH:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][cH:8][c:9]([Br:10])[c:11]1[CH3:12]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][cH:8][c:9]([Br:10])[c:11]1[CH3:12]
CI.Cc1c(Br)cccc1C(=O)O
COC(=O)c1cccc(Br)c1C
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
9474aa79a2adc7353c0c02444ca598a6f486ecdd7ed5edb9ae0645721ee50389
badd4f82161bb0ee7acffd023ea4caae5d036bce7065c10ab0a06e83a6a6f119
c1ccccc1
I-[CH3;D1;+0:1].[O;D1;H0:2]=[C:3](-[OH;D1;+0:4])-[c:5]>>[CH3;D1;+0:1]-[O;H0;D2;+0:4]-[C:3](=[O;D1;H0:2])-[c:5]
103.3
[{"value": 100.0, "product": "BrC=1C(=C(C(=O)OC)C=CC1)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 103.3, "product": "BrC=1C(=C(C(=O)OC)C=CC1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
null
null
A mixture of 3-bromo-2-methylbenzoic acid (16 g, 74.4 mmol), sodium bicarbonate (12.5 g, 148.8 mmol) and iodomethane (21.2 g, 148.8 mmol) in DMF (160 mL) was heated at 60° C. for 2 hours. The mixture was cooled to room temperature and poured into ice water (400 mL). The mixture was extracted with ethyl acetate (4×100 m...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Ester
null
null
c1ccccc1
HI
CN(C)C=O
60
null
CI.Cc1c(Br)cccc1C(=O)O>CN(C)C=O>COC(=O)c1cccc(Br)c1C
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-b650c99db20d4ba6b8fdcb17dc1d1211
COC(=O)c1cccc(Br)c1C.O=C1CCC(=O)N1Br>>COC(=O)c1cccc(Br)c1CBr
BrC=1C(=C(C(=O)OC)C=CC1)C.BrN1C(CCC1=O)=O>>BrC=1C(=C(C(=O)OC)C=CC1)CBr
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][cH:8][c:9]([Br:10])[c:11]1[CH3:12].O=C1CCC(=O)N1[Br:13]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][cH:8][c:9]([Br:10])[c:11]1[CH2:12][Br:13]
COC(=O)c1cccc(Br)c1C.O=C1CCC(=O)N1Br
COC(=O)c1cccc(Br)c1CBr
null
null
C(C)#N
Functional Group Interconversion
Wohl-Ziegler bromination benzyl primary
45c0aca0d63a96f0092e6dded9c888827eaf6379dac179e1cefc99293896300a
08f5e7e34d3f321cce3e85421b38226d6240cca0939494ae61032d4f8405cf22
c1ccccc1
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#8:2]-[C:3](=[O;D1;H0:4])-[c:5]:[c:6](-[CH3;D1;+0:7]):[c:8]>>[#8:2]-[C:3](=[O;D1;H0:4])-[c:5]:[c:6](-[CH2;D2;+0:7]-[Br;H0;D1;+0:1]):[c:8]
107.2
[{"value": 97.0, "product": "BrC=1C(=C(C(=O)OC)C=CC1)CBr", "details": "PERCENTYIELD", "is_desired": false}, {"value": 107.2, "product": "BrC=1C(=C(C(=O)OC)C=CC1)CBr", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of methyl 3-bromo-2-methylbenzoate (17.0 g, 74.22 mmol) and N-bromosuccinimide (15.85 g, 89.06 mmol) in acetonitrile (200 mL) was heated under gently refluxing for 17 hours while a 200 W bulb situated 2 cm away was shining on the reaction flask. The mixture was cooled to room temperature and solvent was remov...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Primary halide
C1CCNC1
null
c1ccccc1
HO-
C(C)#N
null
null
COC(=O)c1cccc(Br)c1C.O=C1CCC(=O)N1Br>C(C)#N>COC(=O)c1cccc(Br)c1CBr
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-c41d82aef6e44542b9d45c4257b7c152
CC(C)(C)OC(=O)[C@@H](N)CCC(N)=O.COC(=O)c1cccc(Br)c1CBr>>CC(C)(C)OC(=O)C(CCC(N)=O)N1Cc2c(Br)cccc2C1=O
C(C)N(CC)CC.BrC=1C(=C(C(=O)OC)C=CC1)CBr.Cl.C(C)(C)(C)OC([C@@H](N)CCC(N)=O)=O>>BrC1=C2CN(C(C2=CC=C1)=O)C(C(=O)OC(C)(C)C)CCC(N)=O
[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[C@H:8]([CH2:9][CH2:10][C:11]([NH2:12])=[O:13])[NH2:14].CO[C:23]([c:22]1[c:16]([CH2:15]Br)[c:17]([Br:18])[cH:19][cH:20][cH:21]1)=[O:24]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH:8]([CH2:9][CH2:10][C:11]([NH2:12])=[O:13])[N:14]1[CH2:15][c:16]2[c:17]([Br:18])[cH:...
CC(C)(C)OC(=O)[C@@H](N)CCC(N)=O.COC(=O)c1cccc(Br)c1CBr
CC(C)(C)OC(=O)C(CCC(N)=O)N1Cc2c(Br)cccc2C1=O
null
null
C1CCOC1
Acylation
OtherReaction
f2ed1ce250db42124a484193f6bf5adb2cca3d127cf7dd7d17db2ebca43fb4a6
0eb062b0407fca631aebf8550994dc507c145d19ea7e1f961f104337865aa8f4
O=C1NCc2ccccc21
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4](-[C;H0;D3;+0:5](=[O;D1;H0:6])-O-C):[c:7].[C;D1;H3:8]-[C:9](-[C;D1;H3:10])(-[C;D1;H3:11])-[#8:12]-[C:13](=[O;D1;H0:14])-[C@@H;D3;+0:15](-[NH2;D1;+0:16])-[C:17]-[C:18]-[C:19](-[N;D1;H2:20])=[O;D1;H0:21]>>[C;D1;H3:8]-[C:9](-[C;D1;H3:10])(-[C;D1;H3:11])-[#8:12]-[C:13](=[O;D1;H0:14])-[CH...
48
[{"value": 48.0, "product": "BrC1=C2CN(C(C2=CC=C1)=O)C(C(=O)OC(C)(C)C)CCC(N)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 47.7, "product": "BrC1=C2CN(C(C2=CC=C1)=O)C(C(=O)OC(C)(C)C)CCC(N)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Triethylamine (4.66 g, 46.09 mmol) was added to a stirred suspension of methyl 3-bromo-2-bromomethylbenzoate (6.45 g, 20.95 mmol) and L-glutamine t-butyl ester hydrochloride (5.0 g, 20.95 mmol) in THF (100 mL). The mixture was heated to reflux for 18 hours. The mixture was cooled to room temperature and solvent was rem...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester.Primary amine
Tertiary amide
null
c1ccc2c(c1)C[NH]C2
c1ccc2c(c1)C[NH]C2
HBr
C1CCOC1
null
null
CC(C)(C)OC(=O)[C@@H](N)CCC(N)=O.COC(=O)c1cccc(Br)c1CBr>C1CCOC1>CC(C)(C)OC(=O)C(CCC(N)=O)N1Cc2c(Br)cccc2C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-cb213946227849cba6cbc5d842b1724b
CC(C)(C)OC(=O)C(CCC(N)=O)N1Cc2c(Br)cccc2C1=O>>CC(C)(C)OC(=O)C(CCC(N)=O)N1Cc2c(C#N)cccc2C1=O
CCOC(=O)C.C(=O)(O)[O-].[Na+].BrC1=C2CN(C(C2=CC=C1)=O)C(C(=O)OC(C)(C)C)CCC(N)=O.CN(C)C=O>>C(#N)C1=C2CN(C(C2=CC=C1)=O)C(C(=O)OC(C)(C)C)CCC(N)=O
Br[c:17]1[c:16]2[c:23]([cH:22][cH:21][cH:20]1)[C:24](=[O:25])[N:14]([CH:8]([C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[CH2:9][CH2:10][C:11]([NH2:12])=[O:13])[CH2:15]2>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH:8]([CH2:9][CH2:10][C:11]([NH2:12])=[O:13])[N:14]1[CH2:15][c:16]2[c:17]([C:18]#[N:19])[cH:20][c...
CC(C)(C)OC(=O)C(CCC(N)=O)N1Cc2c(Br)cccc2C1=O
CC(C)(C)OC(=O)C(CCC(N)=O)N1Cc2c(C#N)cccc2C1=O
null
[Zn].C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd].C1(=CC=CC=C1)P([C-]1C=CC=C1)C1=CC=CC=C1.[C-]1(C=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.[Fe+2]
null
Miscellaneous
OtherReaction
ff84fc4da928bc1dae741694660e3ab081edc2d6809ac065b8295fbc7c4a2cdf
73a96fe5e833259ca394a42f82d6cc2ee7231bcde92d95030d2893b90c3fef76
O=C1NCc2ccccc21
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]1:[c:5]-[C:6](=[O;D1;H0:7])-[#7:8]-[C:9]-1>>[N;D1;H0:10]#[C:11]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]1:[c:5]-[C:6](=[O;D1;H0:7])-[#7:8]-[C:9]-1
74
[{"value": 74.0, "product": "C(#N)C1=C2CN(C(C2=CC=C1)=O)C(C(=O)OC(C)(C)C)CCC(N)=O", "details": "PERCENTYIELD", "is_desired": false}]
120
CELSIUS
null
null
A mixture of tert-butyl 2-(4-bromo-1-oxoisoindolin-2-yl)-4-carbamoylbutanoate (1.2 g, 3.02 mmol), zinc cyamide (0.21 g, 1.81 mmol), tris(dibenzylideneacetone)dipalladium (0.06 g, 0.06 mmol), 1,1′-bis(diphenylphosphino)ferrocene (0.067 g, 0.12 mmol) in deoxygenated DMF (15 mL) was heated to 120° C. under N2 for 6 hours....
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
Nitrile
c1ccc2c(c1)C[NH]C2
c1ccc2c(c1)C[NH]C2
c1ccc2c(c1)C[NH]C2
Br-
[Zn].C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd].C1(=CC=CC=C1)P([C-]1C=CC=C1)C1=CC=CC=C1.[C-]1(C=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.[Fe+2]
120
null
CC(C)(C)OC(=O)C(CCC(N)=O)N1Cc2c(Br)cccc2C1=O>[Zn].C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd].C1(=CC=CC=C1)P([C-]1C=CC=C1)C1=CC=CC=C1.[C-]1(C=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.[Fe+2]>CC(C)(C)OC(=O)C(CCC(N)=O)N1Cc2c(C#N)cccc2C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-04120459d0214e5091aa46bf4c7477b0
CC(C)(C)OC(=O)C(CCC(N)=O)N1Cc2c(C#N)cccc2C1=O>>N#Cc1cccc2c1CN(C(CCC(N)=O)C(=O)O)C2=O
C(#N)C1=C2CN(C(C2=CC=C1)=O)C(C(=O)OC(C)(C)C)CCC(N)=O.FC(C(=O)O)(F)F>>C(#N)C1=C2CN(C(C2=CC=C1)=O)C(C(=O)O)CCC(N)=O
CC(C)(C)[O:19][C:17]([CH:11]([N:10]1[CH2:9][c:8]2[c:3]([C:2]#[N:1])[cH:4][cH:5][cH:6][c:7]2[C:20]1=[O:21])[CH2:12][CH2:13][C:14]([NH2:15])=[O:16])=[O:18]>>[N:1]#[C:2][c:3]1[cH:4][cH:5][cH:6][c:7]2[c:8]1[CH2:9][N:10]([CH:11]([CH2:12][CH2:13][C:14]([NH2:15])=[O:16])[C:17](=[O:18])[OH:19])[C:20]2=[O:21]
CC(C)(C)OC(=O)C(CCC(N)=O)N1Cc2c(C#N)cccc2C1=O
N#Cc1cccc2c1CN(C(CCC(N)=O)C(=O)O)C2=O
null
null
null
Deprotection
Deprotection of carboxylic acid
152e5537e48c95b4a3e767536b0f9f68d1308e5f484070828ab5ed951805157a
7f019d4cfe9b3036d0a2d3a3209aa0e1fcb05418ebee15a4be5e125d315d5f01
O=C1NCc2ccccc21
C-C(-C)(-C)-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
89
[{"value": 89.0, "product": "C(#N)C1=C2CN(C(C2=CC=C1)=O)C(C(=O)O)CCC(N)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 88.5, "product": "C(#N)C1=C2CN(C(C2=CC=C1)=O)C(C(=O)O)CCC(N)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
A mixture of tert-butyl 2-(4-cyano-1-oxoisoindolin-2-yl)-4-carbamoylbutanoate (1.0 g, 2.91 mmol) and trifluoroacetic acid (5 mL) was stirred for 2 hours. The mixture was concentrated and the residue was crystallized from ether (15 mL) to give 2-(4-cyano-1-oxoisoindolin-2-yl)-4-carbamoylbutanoic acid (0.74 g, 89%) as a ...
10.6084/m9.figshare.5104873.v1
null
Ester.Boc
Carboxylic acid
null
null
c1ccc2c(c1)C[NH]C2
Other
null
null
2
CC(C)(C)OC(=O)C(CCC(N)=O)N1Cc2c(C#N)cccc2C1=O>>N#Cc1cccc2c1CN(C(CCC(N)=O)C(=O)O)C2=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-a02a6eb08b5a43b8897cae94a49cff54
N#Cc1cccc2c1CN(C(CCC(N)=O)C(=O)O)C2=O>>N#Cc1cccc2c1CN(C1CCC(=O)NC1=O)C2=O
C(#N)C1=C2CN(C(C2=CC=C1)=O)C(C(=O)O)CCC(N)=O>>O=C1NC(CCC1N1C(C=2C=CC=C(C2C1)C#N)=O)=O
O[C:17]([CH:11]([N:10]1[CH2:9][c:8]2[c:3]([C:2]#[N:1])[cH:4][cH:5][cH:6][c:7]2[C:19]1=[O:20])[CH2:12][CH2:13][C:14](=[O:15])[NH2:16])=[O:18]>>[N:1]#[C:2][c:3]1[cH:4][cH:5][cH:6][c:7]2[c:8]1[CH2:9][N:10]([CH:11]1[CH2:12][CH2:13][C:14](=[O:15])[NH:16][C:17]1=[O:18])[C:19]2=[O:20]
N#Cc1cccc2c1CN(C(CCC(N)=O)C(=O)O)C2=O
N#Cc1cccc2c1CN(C1CCC(=O)NC1=O)C2=O
null
null
C(C)#N
Miscellaneous
OtherReaction
52c2be58e438dca32d8dfc2407dae12033d4d53c2248553cbdbd9b07dc6fc54c
ba17a8a91d881b019f9339558c9ed531b2e73dd4a7c4d7050727d51dac58dc25
O=C1CCC(N2Cc3ccccc3C2=O)C(=O)N1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[#7:4]-[C:5]=[O;D1;H0:6])-[C:7]-[C:8]-[C:9](-[NH2;D1;+0:10])=[O;D1;H0:11]>>[O;D1;H0:11]=[C:9]1-[C:8]-[C:7]-[C:3](-[#7:4]-[C:5]=[O;D1;H0:6])-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:10]-1
83
[{"value": 83.0, "product": "O=C1NC(CCC1N1C(C=2C=CC=C(C2C1)C#N)=O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 78.2, "product": "O=C1NC(CCC1N1C(C=2C=CC=C(C2C1)C#N)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 2-(4-cyano-1-oxoisoindolin-2-yl)-4carbamoylbutanoic acid (0.6 g, 2.09 mmol) and 1,1-carbonyldiimidazole (0.44 g, 2.72 mmol) in acetonitrile (20 mL) was heated to reflux for 2 hours. The mixture was cooled to room temperature and filtered to give 2-(2,6-dioxo(3-piperidyl))-1-oxoisoindoline-4-carbonitrile (0...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amide
Unsubstituted dicarboximide
null
C1CCNCC1
c1ccc2c(c1)C[NH]C2.C1CCNCC1
HO-
C(C)#N
null
null
N#Cc1cccc2c1CN(C(CCC(N)=O)C(=O)O)C2=O>C(C)#N>N#Cc1cccc2c1CN(C1CCC(=O)NC1=O)C2=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-b6604bbee49d413db01a10987e483767
N#Cc1cccc2c1CN(C1CCC(=O)NC1=O)C2=O>>NCc1cccc2c1CN(C1CCC(=O)NC1=O)C2=O
O=C1NC(CCC1N1C(C=2C=CC=C(C2C1)C#N)=O)=O.Cl>>Cl.NCC1=C2CN(C(C2=CC=C1)=O)C1C(NC(CC1)=O)=O
[N:2]#[C:3][c:4]1[cH:5][cH:6][cH:7][c:8]2[c:9]1[CH2:10][N:11]([CH:12]1[CH2:13][CH2:14][C:15](=[O:16])[NH:17][C:18]1=[O:19])[C:20]2=[O:21]>>[NH2:2][CH2:3][c:4]1[cH:5][cH:6][cH:7][c:8]2[c:9]1[CH2:10][N:11]([CH:12]1[CH2:13][CH2:14][C:15](=[O:16])[NH:17][C:18]1=[O:19])[C:20]2=[O:21]
N#Cc1cccc2c1CN(C1CCC(=O)NC1=O)C2=O
NCc1cccc2c1CN(C1CCC(=O)NC1=O)C2=O
null
[Pd]
CO
Reduction
Reduction of nitrile to amine
65bec2d9f430701d30dc9fcbe1c5418f3dfa174d67be035c50edfc71895dc9c7
e8d1bc928b94bd4f5bf4b23363ce8f88b1ce7d146ba93829e7b8ad8dbe0007a7
O=C1CCC(N2Cc3ccccc3C2=O)C(=O)N1
[N;H0;D1;+0:1]#[C;H0;D2;+0:2]-[c:3](:[c:4]):[c:5]>>[NH2;D1;+0:1]-[CH2;D2;+0:2]-[c:3](:[c:4]):[c:5]
99
[{"value": 99.0, "product": "Cl.NCC1=C2CN(C(C2=CC=C1)=O)C1C(NC(CC1)=O)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
17
HOUR
A mixture of 2-(2,6-dioxo(3-piperidyl))-1-oxoisoindoline-4-carbonitrile (1.0 g, 3.71 mmol) and 10% Pd/C (0.2 g) in 4N HCl (20 mL) and methanol (600 mL) was hydrogenated at 50 psi for 17 hours. The mixture was filtered through celite and the filtrate was concentrated. The residue was stirred with ether (30 mL) to give 3...
10.6084/m9.figshare.5104873.v1
null
Nitrile
Primary amine
null
null
c1ccc2c(c1)C[NH]C2.C1CCNCC1
null
[Pd].CO
null
17
N#Cc1cccc2c1CN(C1CCC(=O)NC1=O)C2=O>[Pd].CO>NCc1cccc2c1CN(C1CCC(=O)NC1=O)C2=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-2e0049b47acb409b9843b0b579786509
NCc1cccc2c1CN(C1CCC(=O)NC1=O)C2=O.O=C(Cl)C1CC1>>O=C1CCC(N2Cc3c(CNC(=O)C4CC4)cccc3C2=O)C(=O)N1
N12CCCCCC2=NCCC1.Cl.NCC1=C2CN(C(C2=CC=C1)=O)C1C(NC(CC1)=O)=O.C1(CC1)C(=O)Cl>>O=C1NC(CCC1N1C(C2=CC=CC(=C2C1)CNC(=O)C1CC1)=O)=O
[O:1]=[C:2]1[CH2:3][CH2:4][CH:5]([N:6]2[CH2:7][c:8]3[c:9]([CH2:10][NH2:11])[cH:17][cH:18][cH:19][c:20]3[C:21]2=[O:22])[C:23](=[O:24])[NH:25]1.Cl[C:12](=[O:13])[CH:14]1[CH2:15][CH2:16]1>>[O:1]=[C:2]1[CH2:3][CH2:4][CH:5]([N:6]2[CH2:7][c:8]3[c:9]([CH2:10][NH:11][C:12](=[O:13])[CH:14]4[CH2:15][CH2:16]4)[cH:17][cH:18][cH:19...
NCc1cccc2c1CN(C1CCC(=O)NC1=O)C2=O.O=C(Cl)C1CC1
O=C1CCC(N2Cc3c(CNC(=O)C4CC4)cccc3C2=O)C(=O)N1
null
null
C(C)#N
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
O=C1CCC(N2Cc3c(CNC(=O)C4CC4)cccc3C2=O)C(=O)N1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]1-[C:4]-[C:5]-1.[NH2;D1;+0:6]-[C:7]-[c:8]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[C:7]-[c:8])-[C:3]1-[C:4]-[C:5]-1
50.2
[{"value": 50.0, "product": "O=C1NC(CCC1N1C(C2=CC=CC(=C2C1)CNC(=O)C1CC1)=O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 50.2, "product": "O=C1NC(CCC1N1C(C2=CC=CC(=C2C1)CNC(=O)C1CC1)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
1,8-Diazabicyclo[5,4,0]undec-7-ene (0.7 g, 4.62 mmol) was added to a stirred suspension of 3-[4-(aminomethyl)-1-oxoisoindolin-2-yl]piperidine-2,6-dione hydrochloride (0.65 g, 2.10 mmol) in acetonitrile (50 mL). After stirring for 30 min, cyclopropanecarbonyl chloride (0.24 g, 2.31 mmol) was added. The mixture was stirr...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
C1CCNCC1.C1CC1.c1ccc2c(c1)C[NH]C2
HCl
C(C)#N
null
0.5
NCc1cccc2c1CN(C1CCC(=O)NC1=O)C2=O.O=C(Cl)C1CC1>C(C)#N>O=C1CCC(N2Cc3c(CNC(=O)C4CC4)cccc3C2=O)C(=O)N1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-265838542203460ba52244619f8d3caf
CCN=C=O.NCc1cccc2c1CN(C1CCC(=O)NC1=O)C2=O>>CCNC(=O)NCc1cccc2c1CN(C1CCC(=O)NC1=O)C2=O
N12CCCCCC2=NCCC1.Cl.NCC1=C2CN(C(C2=CC=C1)=O)C1C(NC(CC1)=O)=O.C(C)N=C=O>>O=C1NC(CCC1N1C(C2=CC=CC(=C2C1)CNC(=O)NCC)=O)=O
[CH3:1][CH2:2][N:3]=[C:4]=[O:5].[NH2:6][CH2:7][c:8]1[cH:9][cH:10][cH:11][c:12]2[c:13]1[CH2:14][N:15]([CH:16]1[CH2:17][CH2:18][C:19](=[O:20])[NH:21][C:22]1=[O:23])[C:24]2=[O:25]>>[CH3:1][CH2:2][NH:3][C:4](=[O:5])[NH:6][CH2:7][c:8]1[cH:9][cH:10][cH:11][c:12]2[c:13]1[CH2:14][N:15]([CH:16]1[CH2:17][CH2:18][C:19](=[O:20])[N...
CCN=C=O.NCc1cccc2c1CN(C1CCC(=O)NC1=O)C2=O
CCNC(=O)NCc1cccc2c1CN(C1CCC(=O)NC1=O)C2=O
null
null
C(C)#N
Acylation
Urea synthesis via isocyanate and primary amine
d39cd7dc52a79bb265ff8ef61ef7bf9dc7f7b5fb0150fcb4881bdfb18ab9c380
a5dc801930c765d2a435a0a2973e50163c305ba8e7641d6adbcc1550b7b96de7
O=C1CCC(N2Cc3ccccc3C2=O)C(=O)N1
[C;D1;H3:1]-[C:2]-[N;H0;D2;+0:3]=[C;H0;D2;+0:4]=[O;D1;H0:5].[NH2;D1;+0:6]-[C:7]-[c:8]>>[C;D1;H3:1]-[C:2]-[NH;D2;+0:3]-[C;H0;D3;+0:4](=[O;D1;H0:5])-[NH;D2;+0:6]-[C:7]-[c:8]
42
[{"value": 42.0, "product": "O=C1NC(CCC1N1C(C2=CC=CC(=C2C1)CNC(=O)NCC)=O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 41.9, "product": "O=C1NC(CCC1N1C(C2=CC=CC(=C2C1)CNC(=O)NCC)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
1,8-Diazabicyclo[5,4,0]undec-7-ene (0.44 g, 2.91 mmol) was added to a stirred suspension of 3-[4-(aminomethyl)-1-oxoisoindolin-2-yl]piperidine-2,6-dione hydrochloride (0.6 g, 1.94 mmol) in acetonitrile (50 mL). After stirring for 30 min, ethyl isocyanate (0.21 g, 2.91 mmol) was added. The mixture was stirred at room te...
10.6084/m9.figshare.5104873.v1
null
Isocyanate.Primary amine
Urea
null
null
c1ccc2c(c1)C[NH]C2.C1CCNCC1
null
C(C)#N
null
0.5
CCN=C=O.NCc1cccc2c1CN(C1CCC(=O)NC1=O)C2=O>C(C)#N>CCNC(=O)NCc1cccc2c1CN(C1CCC(=O)NC1=O)C2=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-64b4a14edf7a46439a5c7511642b0ba2
COC(=O)c1c(F)cccc1I.C[C@@H](NC(=O)OC(C)(C)C)c1ccc(B2OC(C)(C)C(C)(C)O2)cc1>>COC(=O)c1c(F)cccc1-c1ccc([C@@H](C)NC(=O)OC(C)(C)C)cc1
CC1(OB(OC1(C)C)C1=CC=C(C=C1)[C@@H](C)NC(OC(C)(C)C)=O)C.FC1=C(C(=O)OC)C(=CC=C1)I.C([O-])([O-])=O.[K+].[K+].C1(=C(C=CC=C1)P(C1=C(C=CC=C1)C)C1=C(C=CC=C1)C)C>>C(C)(C)(C)OC(=O)N[C@H](C)C1=CC=C(C=C1)C=1C(=C(C=CC1)F)C(=O)OC
I[c:11]1[c:5]([C:3]([O:2][CH3:1])=[O:4])[c:6]([F:7])[cH:8][cH:9][cH:10]1.CC1(C)OB([c:12]2[cH:13][cH:14][c:15]([C@@H:16]([CH3:17])[NH:18][C:19](=[O:20])[O:21][C:22]([CH3:23])([CH3:24])[CH3:25])[cH:26][cH:27]2)OC1(C)C>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[c:6]([F:7])[cH:8][cH:9][cH:10][c:11]1-[c:12]1[cH:13][cH:14][c:15]([C@@H...
COC(=O)c1c(F)cccc1I.C[C@@H](NC(=O)OC(C)(C)C)c1ccc(B2OC(C)(C)C(C)(C)O2)cc1
COC(=O)c1c(F)cccc1-c1ccc([C@@H](C)NC(=O)OC(C)(C)C)cc1
null
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-]
C1CCOC1.CCOC(=O)C.O
C-C Coupling
Suzuki coupling with boronic esters
8b44d63590c7228953eb9acb565338c9584155fdcec14c37f9f3f344e065dc2d
b42efb3b6a7742d5af594c6a3031e487327e58e9f8c2f428ee68996c98377910
c1ccc(-c2ccccc2)cc1
C-C1(-C)-O-B(-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5])-O-C-1(-C)-C.I-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9](-[C:10](=[O;D1;H0:11])-[#8:12]-[C;D1;H3:13]):[c:14]>>[C;D1;H3:13]-[#8:12]-[C:10](=[O;D1;H0:11])-[c:9](:[c:14]):[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:7]:[c:8]
18.9
[{"value": 18.9, "product": "C(C)(C)(C)OC(=O)N[C@H](C)C1=CC=C(C=C1)C=1C(=C(C=CC1)F)C(=O)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a stirred solution of tert-butyl (1R)-1-[4-(4,4,5,5-tetramethyl-1,3,2-dioxaborolan-2-yl)phenyl]ethylcarbamate (1.0 g, 2.9 mmol) and methyl 2-fluoro-6-iodobenzoate (1.2 g, 4.32 mmol) in 25 mL of a 5:1 THF:water mixture was added potassium carbonate (1.2 g, 8.64 mmol), tri-o-tolylphosphine (350 mg, 1.15 mmol) and last...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic ester
null
c1ccccc1.B1OCCO1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
HI.B
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].C1CCOC1.CCOC(=O)C.O
null
null
COC(=O)c1c(F)cccc1I.C[C@@H](NC(=O)OC(C)(C)C)c1ccc(B2OC(C)(C)C(C)(C)O2)cc1>C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].C1CCOC1.CCOC(=O)C.O>COC(=O)c1c(F)cccc1-c1ccc([C@@H](C)NC(=O)OC(C)(C)C)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-62a465eb4b2d4de2a03a1d9082e584b5
COC(=O)c1c(F)cccc1-c1ccc([C@@H](C)NC(=O)C2(NC(=O)OC(C)(C)C)CC2)cc1>>C[C@@H](NC(=O)C1(N)CC1)c1ccc(-c2cccc(F)c2C(=O)O)cc1
C(C)(C)(C)OC(=O)NC1(CC1)C(=O)N[C@H](C)C1=CC=C(C=C1)C=1C(=C(C=CC1)F)C(=O)OC>>NC1(CC1)C(=O)N[C@H](C)C1=CC=C(C=C1)C=1C(=C(C=CC1)F)C(=O)O
CC(C)(C)OC(=O)[NH:7][C:6]1([C:4]([NH:3][C@H:2]([CH3:1])[c:10]2[cH:11][cH:12][c:13](-[c:14]3[cH:15][cH:16][cH:17][c:18]([F:19])[c:20]3[C:21](=[O:22])[O:23]C)[cH:24][cH:25]2)=[O:5])[CH2:8][CH2:9]1>>[CH3:1][C@@H:2]([NH:3][C:4](=[O:5])[C:6]1([NH2:7])[CH2:8][CH2:9]1)[c:10]1[cH:11][cH:12][c:13](-[c:14]2[cH:15][cH:16][cH:17][...
COC(=O)c1c(F)cccc1-c1ccc([C@@H](C)NC(=O)C2(NC(=O)OC(C)(C)C)CC2)cc1
C[C@@H](NC(=O)C1(N)CC1)c1ccc(-c2cccc(F)c2C(=O)O)cc1
null
null
C(=O)(C(F)(F)F)O.C(Cl)Cl
Reduction
OtherReaction
45ba1145533a4eb33085691a140a7d6c44cd27a48c5f512bc6db74fad0776eee
227a9aafd021a1d701cc8df6de581eabea9da00b568a3611c608252ac09b2fe2
O=C(NCc1ccc(-c2ccccc2)cc1)C1CC1
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[C:2]1(-[C:3](=[O;D1;H0:4])-[#7:5]-[C:6])-[C:7]-[C:8]-1.C-[O;H0;D2;+0:9]-[C:10](=[O;D1;H0:11])-[c:12]>>[C:6]-[#7:5]-[C:3](=[O;D1;H0:4])-[C:2]1(-[NH2;D1;+0:1])-[C:7]-[C:8]-1.[O;D1;H0:11]=[C:10](-[OH;D1;+0:9])-[c:12]
null
[]
null
null
null
null
A solution of methyl 4′-{(1R)-1-[({1-[(tert-butoxycarbonyl)amino]-cyclopropyl}carbonyl)amino]ethyl}-3-fluoro-1,1′-biphenyl-2-carboxylate (466 mg, 1.0 mmol) in DCM (15 mL) and TFA (15 mL) was stirred under N2 for 20 minutes at ambient temperature, then the organic solvent was removed under vacuum. The residue was dissol...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ester.Ether.Boc
Carboxylic acid.Primary amine
null
null
C1CC1.c1ccccc1.c1ccccc1
HO-
C(=O)(C(F)(F)F)O.C(Cl)Cl
null
null
COC(=O)c1c(F)cccc1-c1ccc([C@@H](C)NC(=O)C2(NC(=O)OC(C)(C)C)CC2)cc1>C(=O)(C(F)(F)F)O.C(Cl)Cl>C[C@@H](NC(=O)C1(N)CC1)c1ccc(-c2cccc(F)c2C(=O)O)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-dd2ed1d732e747bca66ca981bc217465
C[C@@H](NC(=O)C1(N)CC1)c1ccc(-c2cccc(F)c2C(=O)O)cc1.O=C(O)CC(F)(F)F>>C[C@@H](NC(=O)C1(NC(=O)CC(F)(F)F)CC1)c1ccc(-c2cccc(F)c2C(=O)O)cc1
FC(CC(=O)O)(F)F.Cl.C(C)N=C=NCCCN(C)C.ON1N=NC2=C1N=CC=C2.NC1(CC1)C(=O)N[C@H](C)C1=CC=C(C=C1)C=1C(=C(C=CC1)F)C(=O)O.C(C)(C)N(C(C)C)CC>>FC1=C(C(=CC=C1)C1=CC=C(C=C1)[C@@H](C)NC(=O)C1(CC1)NC(CC(F)(F)F)=O)C(=O)O
[CH3:1][C@@H:2]([NH:3][C:4](=[O:5])[C:6]1([NH2:7])[CH2:15][CH2:16]1)[c:17]1[cH:18][cH:19][c:20](-[c:21]2[cH:22][cH:23][cH:24][c:25]([F:26])[c:27]2[C:28](=[O:29])[OH:30])[cH:31][cH:32]1.O[C:8](=[O:9])[CH2:10][C:11]([F:12])([F:13])[F:14]>>[CH3:1][C@@H:2]([NH:3][C:4](=[O:5])[C:6]1([NH:7][C:8](=[O:9])[CH2:10][C:11]([F:12])...
C[C@@H](NC(=O)C1(N)CC1)c1ccc(-c2cccc(F)c2C(=O)O)cc1.O=C(O)CC(F)(F)F
C[C@@H](NC(=O)C1(NC(=O)CC(F)(F)F)CC1)c1ccc(-c2cccc(F)c2C(=O)O)cc1
null
null
C(Cl)Cl
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(NCc1ccc(-c2ccccc2)cc1)C1CC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4](-[F;D1;H0:5])(-[F;D1;H0:6])-[F;D1;H0:7].[C:8]-[#7:9]-[C:10](=[O;D1;H0:11])-[C:12]1(-[NH2;D1;+0:13])-[C:14]-[C:15]-1>>[C:8]-[#7:9]-[C:10](=[O;D1;H0:11])-[C:12]1(-[NH;D2;+0:13]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4](-[F;D1;H0:5])(-[F;D1;H0:6])-[F;D1;H0:7])-[C:14]-[C:15]-1
null
[]
null
null
20
MINUTE
To a solution of trifluoropropionic acid (128 mg, 1.0 mmol) in DCM (1 mL), 1-ethyl-(3-dimethylaminopropyl)carbodiimide hydrochloride (229 mg, 1.2 mmol) and 1-hydroxy-7-azabenzotriazole (136 mg, 1.0 mmol) were added. The resulting solution was stirred at room temperature for 20 minutes, then 4′-((1R)-1-{[(1-aminocyclopr...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
C1CC1.c1ccccc1.c1ccccc1
HO-
C(Cl)Cl
null
0.333333
C[C@@H](NC(=O)C1(N)CC1)c1ccc(-c2cccc(F)c2C(=O)O)cc1.O=C(O)CC(F)(F)F>C(Cl)Cl>C[C@@H](NC(=O)C1(NC(=O)CC(F)(F)F)CC1)c1ccc(-c2cccc(F)c2C(=O)O)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-5ae0c0d393cb48bfbc9062688fae2658
COC(=O)c1ccccc1I.N#Cc1ccc(B(O)O)cc1>>COC(=O)c1ccccc1-c1ccc(C#N)cc1
O.C([O-])([O-])=O.[K+].[K+].IC1=C(C(=O)OC)C=CC=C1.C(#N)C1=CC=C(C=C1)B(O)O>>C(#N)C1=CC=C(C=C1)C=1C(=CC=CC1)C(=O)OC
I[c:10]1[c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:6][cH:7][cH:8][cH:9]1.OB(O)[c:11]1[cH:12][cH:13][c:14]([C:15]#[N:16])[cH:17][cH:18]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][cH:8][cH:9][c:10]1-[c:11]1[cH:12][cH:13][c:14]([C:15]#[N:16])[cH:17][cH:18]1
COC(=O)c1ccccc1I.N#Cc1ccc(B(O)O)cc1
COC(=O)c1ccccc1-c1ccc(C#N)cc1
null
[Pd](Cl)Cl.C1(=C(C=CC=C1)P(C1=C(C=CC=C1)C)C1=C(C=CC=C1)C)C.C1(=C(C=CC=C1)P(C1=C(C=CC=C1)C)C1=C(C=CC=C1)C)C
C1CCOC1
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccccc2)cc1
I-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[C:5](=[O;D1;H0:6])-[#8:7]-[C;D1;H3:8]):[c:9].O-B(-O)-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]>>[C;D1;H3:8]-[#8:7]-[C:5](=[O;D1;H0:6])-[c:4](:[c:9]):[c;H0;D3;+0:1](-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]):[c:2]:[c:3]
86
[{"value": 86.0, "product": "C(#N)C1=CC=C(C=C1)C=1C(=CC=CC1)C(=O)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To 500 mL of THF was added water (18.4 mL, 1.02 mol), potassium carbonate (70.5 g, 0.510 mol), methyl 2-iodobenzoate (53.5 g, 0.204 mol), 4-cyano-phenylboronic acid (30.0 g, 0.204 mol) and bis-(tri-o-tolylphosphine) palladium (II) chloride (1.65 g, 2.04 mmol). This mixture was heated to reflux for 3.5 hours and then co...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
HI.B
[Pd](Cl)Cl.C1(=C(C=CC=C1)P(C1=C(C=CC=C1)C)C1=C(C=CC=C1)C)C.C1(=C(C=CC=C1)P(C1=C(C=CC=C1)C)C1=C(C=CC=C1)C)C.C1CCOC1
null
8
COC(=O)c1ccccc1I.N#Cc1ccc(B(O)O)cc1>[Pd](Cl)Cl.C1(=C(C=CC=C1)P(C1=C(C=CC=C1)C)C1=C(C=CC=C1)C)C.C1(=C(C=CC=C1)P(C1=C(C=CC=C1)C)C1=C(C=CC=C1)C)C.C1CCOC1>COC(=O)c1ccccc1-c1ccc(C#N)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-efb62edd7ac24fc0b072a8bc9da1cb21
COC(=O)c1ccccc1-c1ccc(CNC(=O)C2(NC(=O)OC(C)(C)C)CC2)cc1>>COC(=O)c1ccccc1-c1ccc(CNC(=O)C2(N)CC2)cc1
C(C)(C)(C)OC(=O)NC1(CC1)C(=O)NCC1=CC=C(C=C1)C=1C(=CC=CC1)C(=O)OC.Cl>>NC1(CC1)C(=O)NCC1=CC=C(C=C1)C=1C(=CC=CC1)C(=O)OC
CC(C)(C)OC(=O)[NH:20][C:19]1([C:17]([NH:16][CH2:15][c:14]2[cH:13][cH:12][c:11](-[c:10]3[c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:6][cH:7][cH:8][cH:9]3)[cH:24][cH:23]2)=[O:18])[CH2:21][CH2:22]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][cH:8][cH:9][c:10]1-[c:11]1[cH:12][cH:13][c:14]([CH2:15][NH:16][C:17](=[O:18])[C:19]2([NH...
COC(=O)c1ccccc1-c1ccc(CNC(=O)C2(NC(=O)OC(C)(C)C)CC2)cc1
COC(=O)c1ccccc1-c1ccc(CNC(=O)C2(N)CC2)cc1
null
null
CO.C(Cl)(Cl)Cl.C(Cl)Cl
Reduction
Hydrogenolysis of amides/imides/carbamates
3c33dd2a2d355ee5ba0287367e209aa147a39aa00607f0c95fb2bf1ade45d014
c5b5dffe7dd8beebdc1baa8b5b05300a9f7079e65dcfd42ade6f8a77ff09537d
O=C(NCc1ccc(-c2ccccc2)cc1)C1CC1
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[C:2]1(-[C:3](=[O;D1;H0:4])-[#7:5]-[C:6])-[C:7]-[C:8]-1>>[C:6]-[#7:5]-[C:3](=[O;D1;H0:4])-[C:2]1(-[NH2;D1;+0:1])-[C:7]-[C:8]-1
null
[]
0
CELSIUS
30
MINUTE
Methyl 4′-{[({1-[(tert-butoxycarbonyl)amino]cyclopropyl}carbonyl)-amino]methyl}-1,1′-biphenyl-2-carboxylate (0.84 g, 2.0 mmol) dissolved in a mixture of DCM (3 mL) and MeOH (45 mL) was cooled to 0° C. This homogenous solution was saturated with anhydrous hydrogen chloride and allowed to sit for 30 minutes. Dry nitrogen...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Primary amine
null
null
c1ccccc1.c1ccccc1.C1CC1
HO-
CO.C(Cl)(Cl)Cl.C(Cl)Cl
0
0.5
COC(=O)c1ccccc1-c1ccc(CNC(=O)C2(NC(=O)OC(C)(C)C)CC2)cc1>CO.C(Cl)(Cl)Cl.C(Cl)Cl>COC(=O)c1ccccc1-c1ccc(CNC(=O)C2(N)CC2)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-ea24b883e61146ae966eb07d2c1926f9
CI.COC(=O)c1ccccc1-c1ccc(CNC(=O)C2(N)CC2)cc1>>CNC1(C(=O)NCc2ccc(-c3ccccc3C(=O)OC)cc2)CC1
IC.IC.C(C)N(CC)CC.NC1(CC1)C(=O)NCC1=CC=C(C=C1)C=1C(=CC=CC1)C(=O)OC>>CNC1(CC1)C(=O)NCC1=CC=C(C=C1)C=1C(=CC=CC1)C(=O)OC
I[CH3:1].[NH2:2][C:3]1([C:4](=[O:5])[NH:6][CH2:7][c:8]2[cH:9][cH:10][c:11](-[c:12]3[cH:13][cH:14][cH:15][cH:16][c:17]3[C:18](=[O:19])[O:20][CH3:21])[cH:22][cH:23]2)[CH2:24][CH2:25]1>>[CH3:1][NH:2][C:3]1([C:4](=[O:5])[NH:6][CH2:7][c:8]2[cH:9][cH:10][c:11](-[c:12]3[cH:13][cH:14][cH:15][cH:16][c:17]3[C:18](=[O:19])[O:20][...
CI.COC(=O)c1ccccc1-c1ccc(CNC(=O)C2(N)CC2)cc1
CNC1(C(=O)NCc2ccc(-c3ccccc3C(=O)OC)cc2)CC1
null
null
C(Cl)Cl
Heteroatom Alkylation and Arylation
N-alkylation of primary amines with alkyl halides
3c2788b3f372b76c1d2ee0d77963cb247b210aa8a28e76637b4e731826c4252a
c6874c6af41d3b1c4f7668e1cd342c90252d0e77f4317d31b3193ebc2f9501a3
O=C(NCc1ccc(-c2ccccc2)cc1)C1CC1
I-[CH3;D1;+0:1].[C:2]-[#7:3]-[C:4](=[O;D1;H0:5])-[C:6]1(-[NH2;D1;+0:7])-[C:8]-[C:9]-1>>[C:2]-[#7:3]-[C:4](=[O;D1;H0:5])-[C:6]1(-[NH;D2;+0:7]-[CH3;D1;+0:1])-[C:8]-[C:9]-1
34.8
[{"value": 34.8, "product": "CNC1(CC1)C(=O)NCC1=CC=C(C=C1)C=1C(=CC=CC1)C(=O)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Methyl 4′-({[(1-aminocyclopropyl)carbonyl]amino}methyl)-1,1′-biphenyl-2-carboxylate (200 mg, 0.62 mmol), prepared according to Example 1, was dissolved in 5 mL of DCM along with iodomethane (130 mg, 0.93 mmol) and triethylamine (75 mg, 0.74 mmol). After no reaction was observed at ambient temperature, the reaction mixt...
10.6084/m9.figshare.5104873.v1
null
Primary amine
Secondary amine
null
null
c1ccccc1.c1ccccc1.C1CC1
HI
C(Cl)Cl
null
null
CI.COC(=O)c1ccccc1-c1ccc(CNC(=O)C2(N)CC2)cc1>C(Cl)Cl>CNC1(C(=O)NCc2ccc(-c3ccccc3C(=O)OC)cc2)CC1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-896f0cb194bc4ec183ff7cc5a01dfa5a
O=C(CC(F)(F)F)NC1(C(=O)[O-])CC1>>O=C(CC(F)(F)F)NC1(C(=O)O)CC1
FC(CC(=O)NC1(CC1)C(=O)[O-])(F)F>>FC(CC(=O)NC1(CC1)C(=O)O)(F)F
[O:1]=[C:2]([CH2:3][C:4]([F:5])([F:6])[F:7])[NH:8][C:9]1([C:10](=[O:11])[O-:12])[CH2:13][CH2:14]1>>[O:1]=[C:2]([CH2:3][C:4]([F:5])([F:6])[F:7])[NH:8][C:9]1([C:10](=[O:11])[OH:12])[CH2:13][CH2:14]1
O=C(CC(F)(F)F)NC1(C(=O)[O-])CC1
O=C(CC(F)(F)F)NC1(C(=O)O)CC1
null
null
FC(C(=O)O)(F)F.C(Cl)Cl
Reduction
Carboxylate to carboxylic acid
65edb34f59b888c9ecb87d6c8e9fd76d082de6afc49403d96c457f834c73148e
222e2311064b3cb906d6bdeba44711f5dada050c096bbbcc7b35038975f228e8
C1CC1
[C:1]-[C:2](-[O-;H0;D1:3])=[O;D1;H0:4]>>[C:1]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:3]
null
[]
null
null
3.5
HOUR
tert-Butyl (±)-cis-(acetyloxy)methyl]-1-[(3,3,3-trifluoropropanoyl)-amino]cyclopropane carboxylate (489 mg, 1.44 mmol) was dissolved in a mixture of 4 mL of methylene chloride and 1.22 mL of trifluoroacetic acid. The reaction mixture was allowed to stir at ambient temperature for 3.5 hours. The solvents were removed in...
10.6084/m9.figshare.5104873.v1
null
null
Carboxylic acid
null
null
C1CC1
null
FC(C(=O)O)(F)F.C(Cl)Cl
null
3.5
O=C(CC(F)(F)F)NC1(C(=O)[O-])CC1>FC(C(=O)O)(F)F.C(Cl)Cl>O=C(CC(F)(F)F)NC1(C(=O)O)CC1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-0300c97a88a5417abebd157852f56576
N[C@@]12C[C@H]1COC2=O.O=C(O)CC(F)(F)F>>O=C(CC(F)(F)F)N[C@@]12C[C@H]1COC2=O
C(C)N=C=NCCCN(C)C.N[C@@]12C(OC[C@@H]2C1)=O.FC(CC(=O)O)(F)F.OC1=CC=CC=2NN=NC21>>FC(CC(=O)N[C@@]12C(OC[C@@H]2C1)=O)(F)F
[NH2:8][C@@:9]12[CH2:10][C@H:11]1[CH2:12][O:13][C:14]2=[O:15].O[C:2](=[O:1])[CH2:3][C:4]([F:5])([F:6])[F:7]>>[O:1]=[C:2]([CH2:3][C:4]([F:5])([F:6])[F:7])[NH:8][C@@:9]12[CH2:10][C@H:11]1[CH2:12][O:13][C:14]2=[O:15]
N[C@@]12C[C@H]1COC2=O.O=C(O)CC(F)(F)F
O=C(CC(F)(F)F)N[C@@]12C[C@H]1COC2=O
null
null
O.CN(C=O)C.C(C)N(CC)CC
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C1OC[C@@H]2CC12
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4](-[F;D1;H0:5])(-[F;D1;H0:6])-[F;D1;H0:7].[NH2;D1;+0:8]-[C:9]12-[C:10]-[C:11]-1-[C:12]-[#8:13]-[C:14]-2=[O;D1;H0:15]>>[F;D1;H0:5]-[C:4](-[F;D1;H0:6])(-[F;D1;H0:7])-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:8]-[C:9]12-[C:10]-[C:11]-1-[C:12]-[#8:13]-[C:14]-2=[O;D1;H0:15]
45
[{"value": 45.0, "product": "FC(CC(=O)N[C@@]12C(OC[C@@H]2C1)=O)(F)F", "details": "PERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
(±)-Trans-1-amino-3-oxabicyclo[3.1.0]hexan-2-one (128 mg, 1.13 mmol) was mixed with 3,3,3-trifluoropropionic acid in 2.3 mL of N,N-dimethylformamide. Hydroxybenzotriazole (17.4 mg, 0.11 mmol) was added followed by 1-ethyl-3-(3-dimethylaminopropyl)carbodiimide (282 mg, 1.47 mmol). The pH of the reaction mixture was adju...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
C1OC[C@H]2C[C@@H]12
HO-
O.CN(C=O)C.C(C)N(CC)CC
null
2
N[C@@]12C[C@H]1COC2=O.O=C(O)CC(F)(F)F>O.CN(C=O)C.C(C)N(CC)CC>O=C(CC(F)(F)F)N[C@@]12C[C@H]1COC2=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-816f4cc57baa49938806dfe8822092c7
COC(=O)C(=O)NC1(C(=O)NCc2ccc(-c3cccc(F)c3C(=O)OC)cc2F)CC1.N>>COC(=O)c1c(F)cccc1-c1ccc(CNC(=O)C2(NC(=O)C(N)=O)CC2)c(F)c1
FC1=C(C(=CC=C1)C1=CC(=C(C=C1)CNC(=O)C1(CC1)NC(C(=O)OC)=O)F)C(=O)OC.N>>NC(C(=O)NC1(CC1)C(=O)NCC1=C(C=C(C=C1)C=1C(=C(C=CC1)F)C(=O)OC)F)=O
CO[C:24]([C:22]([NH:21][C:20]1([C:18]([NH:17][CH2:16][c:15]2[cH:14][cH:13][c:12](-[c:11]3[c:5]([C:3]([O:2][CH3:1])=[O:4])[c:6]([F:7])[cH:8][cH:9][cH:10]3)[cH:31][c:29]2[F:30])=[O:19])[CH2:27][CH2:28]1)=[O:23])=[O:26].[NH3:25]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[c:6]([F:7])[cH:8][cH:9][cH:10][c:11]1-[c:12]1[cH:13][cH:14][c...
COC(=O)C(=O)NC1(C(=O)NCc2ccc(-c3cccc(F)c3C(=O)OC)cc2F)CC1.N
COC(=O)c1c(F)cccc1-c1ccc(CNC(=O)C2(NC(=O)C(N)=O)CC2)c(F)c1
null
null
CO.C(Cl)Cl
Acylation
OtherReaction
d5b10d4f469e7a196a3b04a6a9e159a7d90514b6df5b50c1197d4b1b774c04e1
adc0ef6f6c1340dd2dbab737c85bf17fc842769181c5db1a2b4f82b391b28f9f
O=C(NCc1ccc(-c2ccccc2)cc1)C1CC1
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](=[O;D1;H0:4])-[#7:5]-[C:6]-[C:7](-[#7:8])=[O;D1;H0:9].[NH3;D0;+0:10]>>[#7:8]-[C:7](=[O;D1;H0:9])-[C:6]-[#7:5]-[C:3](=[O;D1;H0:4])-[C;H0;D3;+0:1](-[NH2;D1;+0:10])=[O;D1;H0:2]
null
[]
null
null
4
HOUR
To a solution of methyl 3,3′-difluoro-4′-({[(1-{[methoxy(oxo)acetyl]-amino}cyclopropyl)carbonyl]amino}methyl)-1,1′-biphenyl-2-carboxylate (0.02 g, 0.045 mmol, Example 5) in methylene chloride (2 mL) at room temperature was added ammonia (0.224 mL of a 2M solution in methanol, 0.45 mmol). The reaction mixture was stirre...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary amide
null
null
c1ccccc1.c1ccccc1.C1CC1
HO-
CO.C(Cl)Cl
null
4
COC(=O)C(=O)NC1(C(=O)NCc2ccc(-c3cccc(F)c3C(=O)OC)cc2F)CC1.N>CO.C(Cl)Cl>COC(=O)c1c(F)cccc1-c1ccc(CNC(=O)C2(NC(=O)C(N)=O)CC2)c(F)c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-ca7acc999d4a4b90bdd5cd77f7621709
COC(=O)c1ccc(CN(C)c2ccc(CO)cc2)cc1>>c1ccc2c(c1)Cc1ccccc1C2
COC(C1=CC=C(C=C1)CN(C)C1=CC=C(C=C1)CO)=O.CNC.B(Cl)(Cl)Cl.S(O)(O)(=O)=O.[Na+].[Cl-].O>>C1=CC=CC=2CC3=CC=CC=C3CC12
COC(=O)[c:11]1[cH:10][cH:9][c:8]([CH2:7]N(C)[c:4]2[cH:3][cH:2][c:1]([CH2:14]O)[cH:6][cH:5]2)[cH:13][cH:12]1>>[cH:1]1[cH:2][cH:3][c:4]2[c:5]([cH:6]1)[CH2:7][c:8]1[cH:9][cH:10][cH:11][cH:12][c:13]1[CH2:14]2
COC(=O)c1ccc(CN(C)c2ccc(CO)cc2)cc1
c1ccc2c(c1)Cc1ccccc1C2
null
null
C(Cl)Cl
C-C Coupling
OtherReaction
24875f989a02a0e8ed47062214ddf8d1effa61ce7a9813c0d049c846185ed9fd
e277919e1aafa02f374213d4ce654b318607078b6d21fa2b9646a7f1a106a457
c1ccc2c(c1)Cc1ccccc1C2
C-O-C(=O)-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](-[CH2;D2;+0:5]-N(-C)-[c;H0;D3;+0:6]2:[c:7]:[c:8]:[c;H0;D3;+0:9](-[CH2;D2;+0:10]-O):[c:11]:[cH;D2;+0:12]:2):[cH;D2;+0:13]:[c:14]:1>>[CH2;D2;+0:10]1-[c;H0;D3;+0:13]2:[c:14]:[cH;D2;+0:1]:[c:2]:[c:3]:[c:4]:2-[CH2;D2;+0:5]-[c;H0;D3;+0:12]2:[c:11]:[cH;D2;+0:9]:[c:8]:[c:7]:[c;H0;D3;...
null
[]
null
null
8
HOUR
To an ice cold solution of 4-{[(4-hydroxymethyl-phenyl)-methyl-amino]-methyl}-benzoic acid methyl ester (0.5 g, 1.8 mmol) and 3-isopropenyl-phenyl)-dimethyl-amine (0.31 g, 1.9 mmol) in methylene chloride (CH2Cl2, 25 mL)) is added dropwise a solution of boron trichloride (1 M BCl3 in CH2Cl2, 2 mL). The reaction mixture ...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary alcohol.Tertiary amine
null
c1ccccc1.c1ccccc1
c1ccc2c(c1)Cc1ccccc1C2
c1ccc2c(c1)Cc1ccccc1C2
HO-
C(Cl)Cl
null
8
COC(=O)c1ccc(CN(C)c2ccc(CO)cc2)cc1>C(Cl)Cl>c1ccc2c(c1)Cc1ccccc1C2
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-d406d35cc3c140e4a123a0c440055f56
CCNc1cc(O)ccc1C.O=C1OC(=O)c2cccc3cccc1c23>>CCN=c1cc2oc3cc(NCC)c(C)cc3c(-c3cccc4cccc(C(=O)O)c34)c-2cc1C
C(C)NC=1C=C(C=CC1C)O.C1(OC(C2=C3C(C=CC=C13)=CC=C2)=O)=O>>C(C)NC=1C=C2OC3=CC(C(=CC3=C(C2=CC1C)C=1C=CC=C2C=CC=C(C12)C(=O)O)C)=NCC
[CH3:1][CH2:2][NH:3][c:10]1[cH:9][c:8]([OH:7])[cH:17][cH:16][c:14]1[CH3:15].O=[C:13]1[c:19]2[cH:20][cH:21][cH:5][c:23]3[cH:4][cH:25][cH:26][c:27]([c:31]23)[C:28](=[O:29])[O:30]1>>[CH3:1][CH2:2][N:3]=[c:4]1[cH:5][c:6]2[o:7][c:8]3[cH:9][c:10]([NH:11][CH2:12][CH3:13])[c:14]([CH3:15])[cH:16][c:17]3[c:18](-[c:19]3[cH:20][cH...
CCNc1cc(O)ccc1C.O=C1OC(=O)c2cccc3cccc1c23
CCN=c1cc2oc3cc(NCC)c(C)cc3c(-c3cccc4cccc(C(=O)O)c34)c-2cc1C
null
null
S(O)(O)(=O)=O
Aromatic Heterocycle Formation
OtherReaction
eaf25e694d975ade044b44f23f6f6c65eba320d6471b6318df8b5e33ed6c7026
f268f7a9729df6beedb2bc7244fb0bb1587af36ab26414ff5f6af869c9b6e262
N=c1ccc2c(-c3cccc4ccccc34)c3ccccc3oc-2c1
O=[C;H0;D3;+0:1]1-[O;H0;D2;+0:2]-[C:3](=[O;D1;H0:4])-[c:5]2:[c:6]:[cH;D2;+0:7]:[cH;D2;+0:8]:[c;H0;D3;+0:9]3:[cH;D2;+0:10]:[cH;D2;+0:11]:[c:12]:[c;H0;D3;+0:13]-1:[c:14]:2:3.[C;D1;H3:15]-[c:16]1:[c:17]:[cH;D2;+0:18]:[c:19](-[OH;D1;+0:20]):[c:21]:[c;H0;D3;+0:22]:1-[NH;D2;+0:23]-[C:24]-[C;D1;H3:25]>>[C;D1;H3:15]-[c:16]1:[c...
10.8
[{"value": 10.8, "product": "C(C)NC=1C=C2OC3=CC(C(=CC3=C(C2=CC1C)C=1C=CC=C2C=CC=C(C12)C(=O)O)C)=NCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
3-Ethylamino-4-methyl-phenol (0.3 g, 2 mmol) and benzo[de]isochromene-1,3-dione (0.2 g, 1 mmol) in sulfuric acid (3 ml) was heated to 150° C. over a period of 6 h. The reaction mixture was pouring into crushed ice, allowed to stand over a period of 1 h and the precipitate was filtered. The filtrate was neutralized with...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Ester.Ester.Aromatic alcohol.Secondary amine
Carboxylic acid.Secondary amine
c1ccccc1.c1cc2c3c(cccc3c1)COC2
c1ccc2oc3ccccc3cc2c1.c1ccc2ccccc2c1
c1ccc2oc3ccccc3cc2c1.c1ccc2ccccc2c1
null
S(O)(O)(=O)=O
null
1
CCNc1cc(O)ccc1C.O=C1OC(=O)c2cccc3cccc1c23>S(O)(O)(=O)=O>CCN=c1cc2oc3cc(NCC)c(C)cc3c(-c3cccc4cccc(C(=O)O)c34)c-2cc1C
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-be133789f7474c46b372ca0c93b11f4e
COC=CC(=O)OC.N#CCc1ccc(C(F)(F)F)cc1Cl>>COC(=O)CC=C(C#N)c1ccc(C(F)(F)F)cc1Cl
C(CC(O)(C(=O)O)CC(=O)O)(=O)O.CC(C)([O-])C.[Na+].COC=CC(=O)OC.ClC1=C(C=CC(=C1)C(F)(F)F)CC#N>>COC(CC=C(C#N)C1=C(C=C(C=C1)C(F)(F)F)Cl)=O
CO[CH:6]=[CH:5][C:3]([O:2][CH3:1])=[O:4].[CH2:7]([C:8]#[N:9])[c:10]1[cH:11][cH:12][c:13]([C:14]([F:15])([F:16])[F:17])[cH:18][c:19]1[Cl:20]>>[CH3:1][O:2][C:3](=[O:4])[CH2:5][CH:6]=[C:7]([C:8]#[N:9])[c:10]1[cH:11][cH:12][c:13]([C:14]([F:15])([F:16])[F:17])[cH:18][c:19]1[Cl:20]
COC=CC(=O)OC.N#CCc1ccc(C(F)(F)F)cc1Cl
COC(=O)CC=C(C#N)c1ccc(C(F)(F)F)cc1Cl
null
null
O1CCCC1
C-C Coupling
OtherReaction
fdddd73459c44dd061e5b0d164cb9263de91417572ff4635a7371dcacf4bf859
26edb75ca4fecc789f6954d66c05aca32f0909f151ad47629af47ca81bad4cf7
c1ccccc1
C-O-[CH;D2;+0:1]=[CH;D2;+0:2]-[C:3](=[O;D1;H0:4])-[#8:5]-[C;D1;H3:6].[N;D1;H0:7]#[C:8]-[CH2;D2;+0:9]-[c:10](:[c:11]):[c:12]>>[C;D1;H3:6]-[#8:5]-[C:3](=[O;D1;H0:4])-[CH2;D2;+0:2]-[CH;D2;+0:1]=[C;H0;D3;+0:9](-[C:8]#[N;D1;H0:7])-[c:10](:[c:11]):[c:12]
97.3
[{"value": 97.0, "product": "COC(CC=C(C#N)C1=C(C=C(C=C1)C(F)(F)F)Cl)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 97.3, "product": "COC(CC=C(C#N)C1=C(C=C(C=C1)C(F)(F)F)Cl)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
3
HOUR
To a solution of sodium tert-butoxide (3.28 g, 34.2 mmol) in tetrahydrofuran (20 mL) at 0° C. was added a solution of methyl 3-methoxyacrylate (2.65 g, 22.8 mmol) and (2-chloro-4-trifluoromethyl-phenyl)-acetonitrile (5.00 g, 22.8 mmol) in tetrahydrofuran (20 mL) dropwise over 45 minutes. The red solution was stirred at...
10.6084/m9.figshare.5104873.v1
null
Ester.Ether
Ester
null
null
c1ccccc1
HO-
O1CCCC1
0
3
COC=CC(=O)OC.N#CCc1ccc(C(F)(F)F)cc1Cl>O1CCCC1>COC(=O)CC=C(C#N)c1ccc(C(F)(F)F)cc1Cl
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-68c186e6a50c440999f7304d9c1dd3e5
COC=CC(=O)OC.N#CCc1ccccc1Br>>COC(=O)CC=C(C#N)c1ccccc1Br
C(CC(O)(C(=O)O)CC(=O)O)(=O)O.BrC1=C(C=CC=C1)CC#N.COC(C=COC)=O.CC(C)([O-])C.[Na+]>>COC(CC=C(C#N)C1=C(C=CC=C1)Br)=O
CO[CH:6]=[CH:5][C:3]([O:2][CH3:1])=[O:4].[CH2:7]([C:8]#[N:9])[c:10]1[cH:11][cH:12][cH:13][cH:14][c:15]1[Br:16]>>[CH3:1][O:2][C:3](=[O:4])[CH2:5][CH:6]=[C:7]([C:8]#[N:9])[c:10]1[cH:11][cH:12][cH:13][cH:14][c:15]1[Br:16]
COC=CC(=O)OC.N#CCc1ccccc1Br
COC(=O)CC=C(C#N)c1ccccc1Br
null
null
C(C)(C)(C)OC.O1CCCC1
C-C Coupling
OtherReaction
fdddd73459c44dd061e5b0d164cb9263de91417572ff4635a7371dcacf4bf859
26edb75ca4fecc789f6954d66c05aca32f0909f151ad47629af47ca81bad4cf7
c1ccccc1
C-O-[CH;D2;+0:1]=[CH;D2;+0:2]-[C:3](=[O;D1;H0:4])-[#8:5]-[C;D1;H3:6].[N;D1;H0:7]#[C:8]-[CH2;D2;+0:9]-[c:10](:[c:11]):[c:12]>>[C;D1;H3:6]-[#8:5]-[C:3](=[O;D1;H0:4])-[CH2;D2;+0:2]-[CH;D2;+0:1]=[C;H0;D3;+0:9](-[C:8]#[N;D1;H0:7])-[c:10](:[c:11]):[c:12]
99.5
[{"value": 96.0, "product": "COC(CC=C(C#N)C1=C(C=CC=C1)Br)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 99.5, "product": "COC(CC=C(C#N)C1=C(C=CC=C1)Br)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 2-bromo-phenylacetonitrile (6.62 mL, 51.0 mmol) and methyl-3-methoxyacrylate (5.32 mL, 49.5 mmol) in tetrahydrofuran (10 ml) was added to a suspension of sodium tert-butoxide (5.05 g, 51.0 mmol) in tetrahydrofuran (70 mL) at 0° C. over 10 minutes under a stream of nitrogen. The reaction mixture was warmed...
10.6084/m9.figshare.5104873.v1
null
Ester.Ether
Ester
null
null
c1ccccc1
HO-
C(C)(C)(C)OC.O1CCCC1
null
null
COC=CC(=O)OC.N#CCc1ccccc1Br>C(C)(C)(C)OC.O1CCCC1>COC(=O)CC=C(C#N)c1ccccc1Br
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-764b14b9941241a4aa26e7910f5f2e10
CCOC=CC(=O)OCC.N#CCc1ccccc1Br>>N#CC1=CC(=C2OCCO2)c2ccccc21
S(O)(O)(=O)=O.CC(C)([O-])C.[Na+].BrC1=C(C=CC=C1)CC#N.C(C)OC(C=COCC)=O>>O1C(OCC1)=C1C=C(C2=CC=CC=C12)C#N
CC[O:10][C:6]([CH:5]=[CH:4]O[CH2:9][CH3:8])=[O:7].Br[c:11]1[cH:12][cH:13][cH:14][cH:15][c:16]1[CH2:3][C:2]#[N:1]>>[N:1]#[C:2][C:3]1=[CH:4][C:5](=[C:6]2[O:7][CH2:8][CH2:9][O:10]2)[c:11]2[cH:12][cH:13][cH:14][cH:15][c:16]21
CCOC=CC(=O)OCC.N#CCc1ccccc1Br
N#CC1=CC(=C2OCCO2)c2ccccc21
null
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].C1(CCCCC1)P(C1CCCCC1)C1CCCCC1
C(CO)O.O.O1CCCC1
Acylation
OtherReaction
67570292e87e0eca0e7502939e252013a45cf960781d5d135697411d46b48998
95372d00294ac9b4c53a7bcb2b904a19ae3d5134f044b14db9fbb02225bf88fd
C1=Cc2ccccc2C1=C1OCCO1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[CH2;D2;+0:5]-[C:6]#[N;D1;H0:7]):[c:8].C-C-[O;H0;D2;+0:9]-[C;H0;D3;+0:10](=[O;H0;D1;+0:11])-[CH;D2;+0:12]=[CH;D2;+0:13]-O-[CH2;D2;+0:14]-[CH3;D1;+0:15]>>[N;D1;H0:7]#[C:6]-[C;H0;D3;+0:5]1=[CH;D2;+0:13]-[C;H0;D3;+0:12](=[C;H0;D3;+0:10]2-[O;H0;D2;+0:9]-[CH2;D2;+0:14]-[CH2;D2;+0:15]-[...
80
[{"value": 80.0, "product": "O1C(OCC1)=C1C=C(C2=CC=CC=C12)C#N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 79.7, "product": "O1C(OCC1)=C1C=C(C2=CC=CC=C12)C#N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
null
null
A solution of tricyclohexylphosphine (536 mg, 1.91 mmol) in tetrahydrofuran (25 mL) was charged with palladium (II) acetate (287 mg, 1.27 mmol) under nitrogen. After 1 hour the reaction mixture was cooled to 0° C. and charged with sodium tert-butoxide (31.6 g, 319 mmol). After 5 minutes a solution of 2-bromo-phenylacet...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Ether
Ether.Ether
c1ccccc1
C1COCO1.C1=Cc2ccccc2C1
C1COCO1.C1=Cc2ccccc2C1
HBr
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].C1(CCCCC1)P(C1CCCCC1)C1CCCCC1.C(CO)O.O.O1CCCC1
0
null
CCOC=CC(=O)OCC.N#CCc1ccccc1Br>C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].C1(CCCCC1)P(C1CCCCC1)C1CCCCC1.C(CO)O.O.O1CCCC1>N#CC1=CC(=C2OCCO2)c2ccccc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-9aeb12b8ac724711b637d517d0227baf
CCOC=CC(=O)OCC.O=S(=O)(Cc1ccccc1Br)c1ccccc1>>CCOC(=O)C1=CC(S(=O)(=O)c2ccccc2)c2ccccc21
C(C)OC(C=COCC)=O.C1(=CC=CC=C1)S(=O)(=O)CC1=C(C=CC=C1)Br.C1(CCCCC1)P(C1CCCCC1)C1CCCCC1.CC(C)([O-])C.[Na+].P(=O)(O)(O)[O-].[K+]>>C(C)OC(=O)C1=CC(C2=CC=CC=C12)S(=O)(=O)C1=CC=CC=C1
CCO[CH:7]=[CH:6][C:4]([O:3][CH2:2][CH3:1])=[O:5].Br[c:23]1[c:18]([CH2:8][S:9](=[O:10])(=[O:11])[c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[cH:19][cH:20][cH:21][cH:22]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[C:6]1=[CH:7][CH:8]([S:9](=[O:10])(=[O:11])[c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[c:18]2[cH:19][cH:20][cH:21][cH...
CCOC=CC(=O)OCC.O=S(=O)(Cc1ccccc1Br)c1ccccc1
CCOC(=O)C1=CC(S(=O)(=O)c2ccccc2)c2ccccc21
null
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-]
C(C)(C)(C)OC.O1CCCC1
C-C Coupling
OtherReaction
a366f6e85c32623adad474d409e42376af4feda66c2ff117da5b9f19944e3357
c6b9a8d2a5811acd67b90380dc39a63bb1e5eb1730f16ff91844bfb85d364339
O=S(=O)(c1ccccc1)C1C=Cc2ccccc21
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[CH2;D2;+0:5]-[#16:6](=[O;D1;H0:7])(=[O;D1;H0:8])-[c:9]):[c:10].C-C-O-[CH;D2;+0:11]=[CH;D2;+0:12]-[C:13](=[O;D1;H0:14])-[#8:15]-[C:16]>>[C:16]-[#8:15]-[C:13](=[O;D1;H0:14])-[C;H0;D3;+0:12]1=[CH;D2;+0:11]-[CH;D3;+0:5](-[#16:6](=[O;D1;H0:7])(=[O;D1;H0:8])-[c:9])-[c:4](:[c:10]):[c;H0...
85
[{"value": 85.0, "product": "C(C)OC(=O)C1=CC(C2=CC=CC=C12)S(=O)(=O)C1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 84.9, "product": "C(C)OC(=O)C1=CC(C2=CC=CC=C12)S(=O)(=O)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
45
MINUTE
A solution of tricyclohexylphophine (46 mg, 0.164 mmol) in tetrahydrofuran (2.5 mL) under nitrogen was charged with palladium (II) acetate (24.5mg, 0.109 mmol). The reaction mixture was stirred for 45 minutes, then cooled to 0° C. and charged with sodium tert-butoxide (270 mg, 2.73 mmol). After 5 minutes a solution of ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Ether
Ester
c1ccccc1
C1=Cc2ccccc2C1
c1ccccc1.C1=Cc2ccccc2C1
HBr
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].C(C)(C)(C)OC.O1CCCC1
0
0.75
CCOC=CC(=O)OCC.O=S(=O)(Cc1ccccc1Br)c1ccccc1>C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].C(C)(C)(C)OC.O1CCCC1>CCOC(=O)C1=CC(S(=O)(=O)c2ccccc2)c2ccccc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-3ee70e79efcc4788a568601f44073199
CCOC(O)=C1C=C(C#N)c2ccccc21>>CCOC(=O)C1CC(C#N)c2ccccc21
C(=O)O.C(C)OC(=C1C=C(C2=CC=CC=C12)C#N)O.[Na]>>C(C)OC(=O)C1CC(C2=CC=CC=C12)C#N
[CH3:1][CH2:2][O:3][C:4]([OH:5])=[C:6]1[CH:7]=[C:8]([C:9]#[N:10])[c:11]2[cH:12][cH:13][cH:14][cH:15][c:16]21>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]1[CH2:7][CH:8]([C:9]#[N:10])[c:11]2[cH:12][cH:13][cH:14][cH:15][c:16]21
CCOC(O)=C1C=C(C#N)c2ccccc21
CCOC(=O)C1CC(C#N)c2ccccc21
null
[Pd]
C(C)O
Miscellaneous
OtherReaction
06148c76d878034eced412b89c53922e6d73d88da9bad45275ca05942c78ecef
41c21da9fd255f18f2773e8546ef0fb243c5e66ce0c62d14e68cd75fefb1b9e0
c1ccc2c(c1)CCC2
[C:1]-[#8:2]-[C;H0;D3;+0:3](-[OH;D1;+0:4])=[C;H0;D3;+0:5]1-[CH;D2;+0:6]=[C;H0;D3;+0:7](-[C:8]#[N;D1;H0:9])-[c:10](:[c:11]):[c:12]-1:[c:13]>>[C:1]-[#8:2]-[C;H0;D3;+0:3](=[O;H0;D1;+0:4])-[CH;D3;+0:5]1-[CH2;D2;+0:6]-[CH;D3;+0:7](-[C:8]#[N;D1;H0:9])-[c:10](:[c:11]):[c:12]-1:[c:13]
87
[{"value": 87.0, "product": "C(C)OC(=O)C1CC(C2=CC=CC=C12)C#N", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 3-(ethoxy-hydroxy-methylene)-3H-indene-1-carbonitrile, sodium salt, (1.00 g, 4.70 mmol) in ethanol (40 mL) in a pressure reactor was purged with nitrogen for 5 minutes and charged with 5% palladium on carbon (1.00 g, 0.230 mmol) and formic acid (0.180 mL, 4.70 mmol), pH=5 at reaction initiation. The press...
10.6084/m9.figshare.5104873.v1
null
Ether.Enol
Ester
C1=Cc2ccccc2C1
c1ccc2c(c1)CCC2
c1ccc2c(c1)CCC2
null
[Pd].C(C)O
null
null
CCOC(O)=C1C=C(C#N)c2ccccc21>[Pd].C(C)O>CCOC(=O)C1CC(C#N)c2ccccc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-fe9d2c6d13af48da90b699d1f3a1186e
COC(=O)C1CC(CN)c2ccccc21>>O=C1NCC2CC1c1ccccc12
COC(=O)C1CC(C2=CC=CC=C12)CN.CC(C)([O-])C.[Na+]>>O=C1C2C=3C=CC=CC3C(CN1)C2
CO[C:2](=[O:1])[CH:7]1[CH2:6][CH:5]([CH2:4][NH2:3])[c:13]2[c:8]1[cH:9][cH:10][cH:11][cH:12]2>>[O:1]=[C:2]1[NH:3][CH2:4][CH:5]2[CH2:6][CH:7]1[c:8]1[cH:9][cH:10][cH:11][cH:12][c:13]12
COC(=O)C1CC(CN)c2ccccc21
O=C1NCC2CC1c1ccccc12
null
null
CO
Miscellaneous
OtherReaction
574f43f635fc178a747fb62afc76e026e89eb4f966e3ed4a9bd4e8431f774fc2
92bd4402d90a419a2f8338f9414db9222f74d64e606e4b1a47fea24edc8b3ea6
O=C1NCC2CC1c1ccccc12
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[c:4])-[C:5]-[C:6]-[C:7]-[NH2;D1;+0:8]>>[O;D1;H0:2]=[C;H0;D3;+0:1]1-[NH;D2;+0:8]-[C:7]-[C:6]-[C:5]-[C:3]-1-[c:4]
null
[]
null
null
null
null
To a solution of 3-aminomethyl-indan-1-carboxylic acid methyl ester (assume 20.0 mmol, 1 equivalent) in 50 mL of methanol was added 3.84 g of sodium tert-butoxide (40.0 mmol, 2.0 equivalent). The reaction mixture was heated to a reflux for 2 hours. The reaction was cooled to room temperature and concentrated in vacuo. ...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine
Secondary amide
null
c1ccc2c(c1)C1CNCC2C1
c1ccc2c(c1)C1CNCC2C1
HO-
CO
null
null
COC(=O)C1CC(CN)c2ccccc21>CO>O=C1NCC2CC1c1ccccc12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-9ea434e6c09642dfb5cbdfda72b919e8
O=C1NCC2CC1c1ccccc12>>c1ccc2c(c1)C1CNCC2C1
Cl.O=C1C2C=3C=CC=CC3C(CN1)C2.[BH4-].[Na+].O.C1(=CC=C(C=C1)S(=O)(=O)O)C.B(F)(F)F.CCOCC>>S(=O)(=O)(O)C1=CC=C(C)C=C1.C12C=3C=CC=CC3C(CNC1)C2
O=[C:19]1[CH:18]2[c:16]3[c:15]([cH:14][cH:13][cH:12][cH:17]3)[CH:22]([CH2:21][NH:20]1)[CH2:23]2>>[cH:12]1[cH:13][cH:14][c:15]2[c:16]([cH:17]1)[CH:18]1[CH2:19][NH:20][CH2:21][CH:22]2[CH2:23]1
O=C1NCC2CC1c1ccccc12
c1ccc2c(c1)C1CNCC2C1
null
null
CO.O1CCCC1.C(C)(C)O
Reduction
Reduction of secondary amides to amines
ad879f3a74bcad0b9dd5e8fd73398142036862409bd8d4a0c7108821173206e8
ab40188eef2f825df7003af0ffae31d0ce53d126542122535627d3d354cbc9fe
c1ccc2c(c1)C1CNCC2C1
O=[C;H0;D3;+0:1](-[#7:2]-[C:3])-[C:4](-[C:5])-[c:6]>>[C:3]-[#7:2]-[CH2;D2;+0:1]-[C:4](-[C:5])-[c:6]
null
[]
50
CELSIUS
30
MINUTE
To a solution of 1.38 g of 9-oxo-10-aza-tricyclo[6.3.1.02,7]dodeca-2(7),3,5-triene (8.00 mmol, 1 equivalent) in 8 mL of tetrahydrofuran was added 603 mg of sodium borohydride (16.0 mmol, 2.0 equivalent) followed by slow addition of 2.77 mL of boron trifluoride diethyl etherate (21.6 mmol, 2.7 equivalent). Once the effe...
10.6084/m9.figshare.5104873.v1
null
Secondary amide
null
c1ccc2c(c1)C1CNCC2C1
c1ccc2c(c1)C1CNCC2C1
c1ccc2c(c1)C1CNCC2C1
Other
CO.O1CCCC1.C(C)(C)O
50
0.5
O=C1NCC2CC1c1ccccc12>CO.O1CCCC1.C(C)(C)O>c1ccc2c(c1)C1CNCC2C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-f50af6e907c34b0d9fd2e41cc802c21a
O=C(N1CC2CC(C1)c1ccccc12)C(F)(F)F.O=[N+]([O-])O>>O=C(N1CC2CC(C1)c1cc([N+](=O)[O-])ccc12)C(F)(F)F
[N+](=O)(O)[O-].FC(S(=O)(=O)O)(F)F.C12C=3C=CC=CC3C(CN(C1)C(C(F)(F)F)=O)C2>>[N+](=O)([O-])C1=CC=2C3CN(CC(C2C=C1)C3)C(C(F)(F)F)=O
[O:1]=[C:2]([N:3]1[CH2:4][CH:5]2[CH2:6][CH:7]([CH2:8]1)[c:9]1[cH:10][cH:11][cH:15][cH:16][c:17]12)[C:18]([F:19])([F:20])[F:21].O[N+:12](=[O:13])[O-:14]>>[O:1]=[C:2]([N:3]1[CH2:4][CH:5]2[CH2:6][CH:7]([CH2:8]1)[c:9]1[cH:10][c:11]([N+:12](=[O:13])[O-:14])[cH:15][cH:16][c:17]12)[C:18]([F:19])([F:20])[F:21]
O=C(N1CC2CC(C1)c1ccccc12)C(F)(F)F.O=[N+]([O-])O
O=C(N1CC2CC(C1)c1cc([N+](=O)[O-])ccc12)C(F)(F)F
null
null
C(Cl)Cl
Functional Group Addition
Aromatic nitration with HNO3
fbc183fc1c4671a7888d30681094affb85dfa1112d21be8a1cb6254bb6af1b07
ddce49825c02b8965f10c8d99e3c841d26e1f136da6037b417c09313e6d73097
c1ccc2c(c1)C1CNCC2C1
O-[N+;H0;D3:1](-[O;-;D1;H0:2])=[O;D1;H0:3].[c:4]:[c:5]:[cH;D2;+0:6]:[c:7]:[c:8]>>[O;-;D1;H0:2]-[N+;H0;D3:1](=[O;D1;H0:3])-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:5]:[c:4]
78
[{"value": 78.0, "product": "[N+](=O)([O-])C1=CC=2C3CN(CC(C2C=C1)C3)C(C(F)(F)F)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 77.8, "product": "[N+](=O)([O-])C1=CC=2C3CN(CC(C2C=C1)C3)C(C(F)(F)F)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-78
CELSIUS
30
MINUTE
(Based on the method described by Coon, C. L.; Blucher, W. G.; Hill, M. E. J. Org. Chem. 1973, 25, 4243.) To a solution of trifluoromethanesulfonic acid (2.4 ml, 13.7 mmol) in CH2Cl2 (10 ml) stirred at 0° C. was slowly added nitric acid (0.58 ml, 27.4 mmol) generating a white precipitate. After 10 minutes the resulting...
10.6084/m9.figshare.5104873.v1
null
Nitrate
Nitro group
c1ccc2c(c1)C1C[NH]CC2C1
c1ccc2c(c1)C1C[NH]CC2C1
c1ccc2c(c1)C1C[NH]CC2C1
HO-
C(Cl)Cl
-78
0.5
O=C(N1CC2CC(C1)c1ccccc12)C(F)(F)F.O=[N+]([O-])O>C(Cl)Cl>O=C(N1CC2CC(C1)c1cc([N+](=O)[O-])ccc12)C(F)(F)F
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-6dc5260fbcaf4265958a4eac66912ab7
O=C(N1CC2CC(C1)c1cc([N+](=O)[O-])ccc12)C(F)(F)F>>Nc1ccc2c(c1)C1CC2CN(C(=O)C(F)(F)F)C1
[N+](=O)([O-])C1=CC=2C3CN(CC(C2C=C1)C3)C(C(F)(F)F)=O>>NC1=CC=2C3CN(CC(C2C=C1)C3)C(C(F)(F)F)=O
O=[N+:1]([O-])[c:2]1[cH:3][cH:4][c:5]2[c:6]([cH:7]1)[CH:8]1[CH2:9][CH:10]2[CH2:11][N:12]([C:13](=[O:14])[C:15]([F:16])([F:17])[F:18])[CH2:19]1>>[NH2:1][c:2]1[cH:3][cH:4][c:5]2[c:6]([cH:7]1)[CH:8]1[CH2:9][CH:10]2[CH2:11][N:12]([C:13](=[O:14])[C:15]([F:16])([F:17])[F:18])[CH2:19]1
O=C(N1CC2CC(C1)c1cc([N+](=O)[O-])ccc12)C(F)(F)F
Nc1ccc2c(c1)C1CC2CN(C(=O)C(F)(F)F)C1
null
[Pd]
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc2c(c1)C1CNCC2C1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
94.5
[{"value": 94.5, "product": "NC1=CC=2C3CN(CC(C2C=C1)C3)C(C(F)(F)F)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Hydrogenation of 1-(4-nitro-10-aza-tricyclo[6.3.1.02,7]dodeca-2(7),3,5-trien-10-yl)-2,2,2-trifluoro-ethanone (2.0 g, 6.66 mmol) under a hydrogen atmosphere (40 psi, or approximately 2.7 atmospheres) and 10% Pd/C (200 mg) in methanol over 1.5 hours, filtration through Celite and concentration affords a yellow oil (1.7 g...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccc2c(c1)C1C[NH]CC2C1
Other
[Pd].CO
null
null
O=C(N1CC2CC(C1)c1cc([N+](=O)[O-])ccc12)C(F)(F)F>[Pd].CO>Nc1ccc2c(c1)C1CC2CN(C(=O)C(F)(F)F)C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-bcb560618ed647df924c3601e43a5253
O=C(N1CC2CC(C1)c1cc([N+](=O)[O-])c([N+](=O)[O-])cc12)C(F)(F)F>>O=[N+]([O-])c1cc2c(cc1[N+](=O)[O-])C1CNCC2C1
CO.C(Cl)Cl.[N+](=O)([O-])C1=CC=2C3CN(CC(C2C=C1[N+](=O)[O-])C3)C(C(F)(F)F)=O.C(=O)([O-])[O-].[Na+].[Na+].O>>[N+](=O)([O-])C1=CC=2C3CNCC(C2C=C1[N+](=O)[O-])C3
O=C(C(F)(F)F)[N:15]1[CH2:14][CH:13]2[c:7]3[c:6]([cH:5][c:4]([N+:2](=[O:1])[O-:3])[c:9]([N+:10](=[O:11])[O-:12])[cH:8]3)[CH:17]([CH2:16]1)[CH2:18]2>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][c:6]2[c:7]([cH:8][c:9]1[N+:10](=[O:11])[O-:12])[CH:13]1[CH2:14][NH:15][CH2:16][CH:17]2[CH2:18]1
O=C(N1CC2CC(C1)c1cc([N+](=O)[O-])c([N+](=O)[O-])cc12)C(F)(F)F
O=[N+]([O-])c1cc2c(cc1[N+](=O)[O-])C1CNCC2C1
null
null
CO
Reduction
Hydrogenolysis of tertiary amines
f46cbee729057ebd415120d06c8d35552e9f6cc6e71a027737f358de057e1ec8
9d0759623d33e2d41aafe1af3bb1025d4d7a88f20060c872279b889c110cab65
c1ccc2c(c1)C1CNCC2C1
F-C(-F)(-F)-C(=O)-[N;H0;D3;+0:1](-[C:2]-[C:3])-[C:4]-[C:5]>>[C:3]-[C:2]-[NH;D2;+0:1]-[C:4]-[C:5]
null
[]
null
null
null
null
1-(4,5-Dinitro-10-aza-tricyclo[6.3.1.02,7]dodeca-2(7),3,5-trien-10-yl)-2,2,2-trifluoro-ethanone (3.7 g, 10.7 mmol) and Na2CO3 (2.3 g, 21.4 mmol) were combined in methanol (50 mL) and H2O (20 mL) then warmed to reflux for 18 hours. The reaction was cooled, concentrated, treated with H2O and extracted with CH2Cl2 (3×50 m...
10.6084/m9.figshare.5104873.v1
null
Trifluoro group.Tertiary amide
Secondary amine
c1ccc2c(c1)C1C[NH]CC2C1
c1ccc2c(c1)C1CNCC2C1
c1ccc2c(c1)C1CNCC2C1
Other
CO
null
null
O=C(N1CC2CC(C1)c1cc([N+](=O)[O-])c([N+](=O)[O-])cc12)C(F)(F)F>CO>O=[N+]([O-])c1cc2c(cc1[N+](=O)[O-])C1CNCC2C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-0c19ea09f0b842fa85fbf56d92b2f314
CC(C)(C)OC(=O)N1CC2CC(C1)c1cc([N+](=O)[O-])c([N+](=O)[O-])cc12>>CC(C)(C)OC(=O)N1CC2CC(C1)c1cc(N)c(N)cc12
C(C)(C)(C)OC(=O)N1CC2C=3C=C(C(=CC3C(C1)C2)[N+](=O)[O-])[N+](=O)[O-]>>C(C)(C)(C)OC(=O)N1CC2C=3C=C(C(=CC3C(C1)C2)N)N
O=[N+:17]([O-])[c:16]1[cH:15][c:14]2[c:21]([cH:20][c:18]1[N+:19](=O)[O-])[CH:10]1[CH2:9][N:8]([C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[CH2:13][CH:12]2[CH2:11]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[N:8]1[CH2:9][CH:10]2[CH2:11][CH:12]([CH2:13]1)[c:14]1[cH:15][c:16]([NH2:17])[c:18]([NH2:19])[cH:20][c...
CC(C)(C)OC(=O)N1CC2CC(C1)c1cc([N+](=O)[O-])c([N+](=O)[O-])cc12
CC(C)(C)OC(=O)N1CC2CC(C1)c1cc(N)c(N)cc12
null
[Pd]
CO
Reduction
OtherReaction
6748a51a25102225412593c5a930e43f5a8904a80803177de025a6f83c59d65e
a303b0dfb15cc6bade463acf71681cf3ba7580b599dfa4d28d8caac83d08cd17
c1ccc2c(c1)C1CNCC2C1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4](-[N+;H0;D3:5](=O)-[O-]):[c:6]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4](-[NH2;D1;+0:5]):[c:6]
null
[]
null
null
null
null
4,5-Dinitro-10-aza-tricyclo[6.3.1.02,7]dodeca-2(7),3,5-triene-10-carboxylic acid tert-butyl ester (1.9 g, 5.44 mmol) was hydrogenated in methanol under a H2 atmosphere (45 psi, or approximately 3 atmospheres) over 10% Pd/C (100 mg) for 1.5 hours then filtered through a Celite pad and concentrated to white solids (1.57 ...
10.6084/m9.figshare.5104873.v1
null
Nitro group.Nitro group
Primary amine.Primary amine
null
null
c1ccc2c(c1)C1C[NH]CC2C1
Other
[Pd].CO
null
null
CC(C)(C)OC(=O)N1CC2CC(C1)c1cc([N+](=O)[O-])c([N+](=O)[O-])cc12>[Pd].CO>CC(C)(C)OC(=O)N1CC2CC(C1)c1cc(N)c(N)cc12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-c87a28432656476ca44431e7feb16a78
CCCI.Cc1nc2cc3c(cc2[nH]1)C1CC3CN(C(=O)OC(C)(C)C)C1>>CCCn1c(C)nc2cc3c(cc21)C1CC3CN(C(=O)OC(C)(C)C)C1
O.CS(=O)C.ICCC.C(C)(C)(C)OC(=O)N1CC2C=3C=C4NC(=NC4=CC3C(C1)C2)C>>C(C)(C)(C)OC(=O)N1CC2C=3C=C4N(C(=NC4=CC3C(C1)C2)C)CCC
I[CH2:3][CH2:2][CH3:1].[nH:4]1[c:5]([CH3:6])[n:7][c:8]2[cH:9][c:10]3[c:11]([cH:12][c:13]12)[CH:14]1[CH2:15][CH:16]3[CH2:17][N:18]([C:19](=[O:20])[O:21][C:22]([CH3:23])([CH3:24])[CH3:25])[CH2:26]1>>[CH3:1][CH2:2][CH2:3][n:4]1[c:5]([CH3:6])[n:7][c:8]2[cH:9][c:10]3[c:11]([cH:12][c:13]12)[CH:14]1[CH2:15][CH:16]3[CH2:17][N:...
CCCI.Cc1nc2cc3c(cc2[nH]1)C1CC3CN(C(=O)OC(C)(C)C)C1
CCCn1c(C)nc2cc3c(cc21)C1CC3CN(C(=O)OC(C)(C)C)C1
null
null
CO.C(Cl)Cl.[OH-].[Na+]
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
aad23a87a709faa184cade5ee8ef98668cac9bd08b2cae918b7a2312b85c430e
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1nc2cc3c(cc2[nH]1)C1CNCC3C1
I-[CH2;D2;+0:1]-[C:2]-[C;D1;H3:3].[C;D1;H3:4]-[c:5]1:[#7;a:6]:[c:7](:[c:8]):[c:9](:[c:10]):[nH;D2;+0:11]:1>>[C;D1;H3:3]-[C:2]-[CH2;D2;+0:1]-[n;H0;D3;+0:11]1:[c:9](:[c:10]):[c:7](:[c:8]):[#7;a:6]:[c:5]:1-[C;D1;H3:4]
null
[]
40
CELSIUS
null
null
(For conditions, see; Pilarski, B. Liebigs Ann. Chem. 1983, 1078.) 6-Methyl-5,7,13-triazatetracyclo[9.3.1.02,10.04,8]pentadeca-2(10),3,5,8-tetraene-13-carboxylic acid tert-butyl ester (80 mg, 0.267 mmol) was stirred in 50% aqueous NaOH solution (3 mL) and DMSO (1 mL) then treated with 1-iodopropane (0.03 mL, 0.321 mmol...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1nc2cc3c(cc2[nH]1)C1C[NH]CC3C1
c1nc2cc3c(cc2[nH]1)C1CNCC3C1
c1nc2cc3c(cc2[nH]1)C1CNCC3C1
HI
CO.C(Cl)Cl.[OH-].[Na+]
40
null
CCCI.Cc1nc2cc3c(cc2[nH]1)C1CC3CN(C(=O)OC(C)(C)C)C1>CO.C(Cl)Cl.[OH-].[Na+]>CCCn1c(C)nc2cc3c(cc21)C1CC3CN(C(=O)OC(C)(C)C)C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-f83b060476964130952cd72d63482d88
CCCn1c(C)nc2cc3c(cc21)C1CC3CN(C(=O)OC(C)(C)C)C1>>CCCn1c(C)nc2cc3c(cc21)C1CNCC3C1
C(C)(C)(C)OC(=O)N1CC2C=3C=C4N(C(=NC4=CC3C(C1)C2)C)CCC.C(C)(=O)OCC.Cl>>Cl.CC1=NC2=CC=3C4CNCC(C3C=C2N1CCC)C4
CC(C)(C)OC(=O)[N:16]1[CH2:15][CH:14]2[c:11]3[c:10]([cH:9][c:8]4[n:7][c:5]([CH3:6])[n:4]([CH2:3][CH2:2][CH3:1])[c:13]4[cH:12]3)[CH:18]([CH2:17]1)[CH2:19]2>>[CH3:1][CH2:2][CH2:3][n:4]1[c:5]([CH3:6])[n:7][c:8]2[cH:9][c:10]3[c:11]([cH:12][c:13]12)[CH:14]1[CH2:15][NH:16][CH2:17][CH:18]3[CH2:19]1
CCCn1c(C)nc2cc3c(cc21)C1CC3CN(C(=O)OC(C)(C)C)C1
CCCn1c(C)nc2cc3c(cc21)C1CNCC3C1
null
null
null
Reduction
Boc amine deprotection
dcd46ab88030f5ae0f98a0a8c5055b6f1f961ba3f911435fc414afcbf6254310
a94b29c7264c852156fc1cdd4a0951a4fc26c06d0edc9e50c743825dbf79e3fd
c1nc2cc3c(cc2[nH]1)C1CNCC3C1
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1](-[C:2]-[C:3])-[C:4]-[C:5]>>[C:3]-[C:2]-[NH;D2;+0:1]-[C:4]-[C:5]
34
[{"value": 34.0, "product": "Cl.CC1=NC2=CC=3C4CNCC(C3C=C2N1CCC)C4", "details": "PERCENTYIELD", "is_desired": false}]
100
CELSIUS
null
null
6-Methyl-7-propyl-5,7,13-triazatetracyclo[9.3.1.02,10.04,8]pentadeca-2(10),3,5,8-tetraene-13-carboxylic acid tert-butyl ester (90 mg, 0.253 mmol) was dissolved in 3N HCl ethyl acetate (5 mL) and warmed to 100° C. for ½ hour. The mixture was cooled, concentrated, slurried in ethyl acetate, and filtered to provide a whit...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Secondary amine
c1nc2cc3c(cc2n1)C1CNCC3C1
c1nc2cc3c(cc2[nH]1)C1CNCC3C1
c1nc2cc3c(cc2[nH]1)C1CNCC3C1
HO-
null
100
null
CCCn1c(C)nc2cc3c(cc21)C1CC3CN(C(=O)OC(C)(C)C)C1>>CCCn1c(C)nc2cc3c(cc21)C1CNCC3C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-931bc6064bc349a4bd207d7c42a61231
CCCCNc1cc2c(cc1[N+](=O)[O-])C1CC2CN(C(=O)OC(C)(C)C)C1>>CCCCNc1cc2c(cc1N)C1CC2CN(C(=O)OC(C)(C)C)C1
C(C)(C)(C)OC(=O)N1CC2C=3C=C(C(=CC3C(C1)C2)NCCCC)[N+](=O)[O-].C(=O)[O-].[NH4+]>>C(C)(C)(C)OC(=O)N1CC2C=3C=C(C(=CC3C(C1)C2)NCCCC)N
O=[N+:12]([O-])[c:11]1[c:6]([NH:5][CH2:4][CH2:3][CH2:2][CH3:1])[cH:7][c:8]2[c:9]([cH:10]1)[CH:13]1[CH2:14][CH:15]2[CH2:16][N:17]([C:18](=[O:19])[O:20][C:21]([CH3:22])([CH3:23])[CH3:24])[CH2:25]1>>[CH3:1][CH2:2][CH2:3][CH2:4][NH:5][c:6]1[cH:7][c:8]2[c:9]([cH:10][c:11]1[NH2:12])[CH:13]1[CH2:14][CH:15]2[CH2:16][N:17]([C:1...
CCCCNc1cc2c(cc1[N+](=O)[O-])C1CC2CN(C(=O)OC(C)(C)C)C1
CCCCNc1cc2c(cc1N)C1CC2CN(C(=O)OC(C)(C)C)C1
null
[OH-].[OH-].[Pd+2]
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc2c(c1)C1CNCC2C1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
100.3
[{"value": 100.0, "product": "C(C)(C)(C)OC(=O)N1CC2C=3C=C(C(=CC3C(C1)C2)NCCCC)N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 100.3, "product": "C(C)(C)(C)OC(=O)N1CC2C=3C=C(C(=CC3C(C1)C2)NCCCC)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
4-Butylamino-5-nitro-10-aza-tricyclo[6.3.1.02,7]dodeca-2(7),3,5-triene-10-carboxlic acid tert-butyl ester (460 mg, 1.27 mmol) was treated with ammonium formate (850 mg, 12.7 mmol) and 10%Pd(OH)2/C (50 mg) in methanol (20 mL) and brought to reflux for 1 hour then filtered through a Celite pad and concentrated. The solid...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccc2c(c1)C1C[NH]CC2C1
Other
[OH-].[OH-].[Pd+2].CO
null
null
CCCCNc1cc2c(cc1[N+](=O)[O-])C1CC2CN(C(=O)OC(C)(C)C)C1>[OH-].[OH-].[Pd+2].CO>CCCCNc1cc2c(cc1N)C1CC2CN(C(=O)OC(C)(C)C)C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-5fd698ef781248f897af3e0a916d0162
CCCCNc1cc2c(cc1N)C1CC2CN(C(=O)OC(C)(C)C)C1>>CCCCn1cnc2cc3c(cc21)C1CC3CN(C(=O)OC(C)(C)C)C1
CO.C(Cl)Cl.CC(=O)O.C(C)OC=C(C#N)C#N.C(C)(C)(C)OC(=O)N1CC2C=3C=C(C(=CC3C(C1)C2)NCCCC)N>>C(C)(C)(C)OC(=O)N1CC2C=3C=C4N(C=NC4=CC3C(C1)C2)CCCC
[CH3:1][CH2:2][CH2:3][CH2:4][NH:5][c:13]1[c:8]([NH2:7])[cH:9][c:11]2[c:10]([cH:12]1)[CH:16]1[CH2:15][CH:14]2[CH2:26][N:18]([C:19](=[O:20])[O:21][C:22]([CH3:23])([CH3:24])[CH3:25])[CH2:17]1>>[CH3:1][CH2:2][CH2:3][CH2:4][n:5]1[cH:6][n:7][c:8]2[cH:9][c:10]3[c:11]([cH:12][c:13]12)[CH:14]1[CH2:15][CH:16]3[CH2:17][N:18]([C:1...
CCCCNc1cc2c(cc1N)C1CC2CN(C(=O)OC(C)(C)C)C1
CCCCn1cnc2cc3c(cc21)C1CC3CN(C(=O)OC(C)(C)C)C1
null
null
C(C)O
Aromatic Heterocycle Formation
OtherReaction
58e4d4c9d07ce70a4dd58e6fc4c563bacf7e98649eca2489fa926dfb4a14e612
c12bf4e666f812d0e692aca3756678364265d1c8b3469e9563c84f9ed1df94d2
c1nc2cc3c(cc2[nH]1)C1CNCC3C1
[C:1]-[C:2]-[NH;D2;+0:3]-[c:4]1:[cH;D2;+0:5]:[c;H0;D3;+0:6]2:[c;H0;D3;+0:7](:[cH;D2;+0:8]:[c:9]:1-[NH2;D1;+0:10])-[C:11]1-[C:12]-[C:13]-2-[C:14]-[#7:15]-[C:16]-1>>[C:1]-[C:2]-[n;H0;D3;+0:3]1:[c:17]:[n;H0;D2;+0:10]:[c:9]2:[cH;D2;+0:8]:[c;H0;D3;+0:6]3:[c;H0;D3;+0:7](:[cH;D2;+0:5]:[c:4]:2:1)-[C:11]1-[C:12]-[C:13]-3-[C:14]...
null
[]
60
CELSIUS
18
HOUR
4-Butylamino-5-amino-10-aza-tricyclo[6.3.1.02,7]dodeca-2(7),3,5-triene-10-carboxylic acid tert-butyl ester (440 mg, 1.27 mmol) was dissolved in ethanol (20 mL) and HOAc (2 mL) and treated with ethoxymethylenemalononitrile (186 mg, 1.52 mmol). The resulting mixture was warmed to 60° C. and stirred 18 hours. The reaction...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Secondary amine
null
c1ccc2c(c1)C1C[NH]CC2C1
c1nc2cc3c(cc2[nH]1)C1CNCC3C1
c1nc2cc3c(cc2[nH]1)C1CNCC3C1
Other
C(C)O
60
18
CCCCNc1cc2c(cc1N)C1CC2CN(C(=O)OC(C)(C)C)C1>C(C)O>CCCCn1cnc2cc3c(cc21)C1CC3CN(C(=O)OC(C)(C)C)C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-69507ca7e21845ed9a875238fec81819
CC(=O)O.CC(C)CNc1cc2c(cc1N)C1CC2CN(C(=O)OC(C)(C)C)C1>>Cc1nc2cc3c(cc2n1CC(C)C)C1CC3CN(C(=O)OC(C)(C)C)C1
CO.C(Cl)Cl.CC(=O)O.C(C)(C)(C)OC(=O)N1CC2C=3C=C(C(=CC3C(C1)C2)N)NCC(C)C>>C(C)(C)(C)OC(=O)N1CC2C=3C=C4N(C(=NC4=CC3C(C1)C2)C)CC(C)C
O=[C:2](O)[CH3:1].[NH2:3][c:4]1[cH:5][c:7]2[c:6]([cH:8][c:9]1[NH:10][CH2:11][CH:12]([CH3:13])[CH3:14])[CH:17]1[CH2:16][CH:15]2[CH2:27][N:19]([C:20](=[O:21])[O:22][C:23]([CH3:24])([CH3:25])[CH3:26])[CH2:18]1>>[CH3:1][c:2]1[n:3][c:4]2[cH:5][c:6]3[c:7]([cH:8][c:9]2[n:10]1[CH2:11][CH:12]([CH3:13])[CH3:14])[CH:15]1[CH2:16][...
CC(=O)O.CC(C)CNc1cc2c(cc1N)C1CC2CN(C(=O)OC(C)(C)C)C1
Cc1nc2cc3c(cc2n1CC(C)C)C1CC3CN(C(=O)OC(C)(C)C)C1
null
null
C(C)O
Aromatic Heterocycle Formation
OtherReaction
147bd722a7163a98731b13d4d837c181454bc91a562ab6f1acf8f083a0edef14
2c7e28df6187a1559bf3bdf429be12550f69083c743a14154a096b0d7c5276e7
c1nc2cc3c(cc2[nH]1)C1CNCC3C1
O-[C;H0;D3;+0:1](=O)-[C;D1;H3:2].[C:3]-[C:4]-[NH;D2;+0:5]-[c:6]1:[cH;D2;+0:7]:[c;H0;D3;+0:8]2:[c;H0;D3;+0:9](:[cH;D2;+0:10]:[c:11]:1-[NH2;D1;+0:12])-[C:13]1-[C:14]-[C:15]-2-[C:16]-[#7:17]-[C:18]-1>>[C:3]-[C:4]-[n;H0;D3;+0:5]1:[c:6]2:[cH;D2;+0:7]:[c;H0;D3;+0:9]3:[c;H0;D3;+0:8](:[cH;D2;+0:10]:[c:11]:2:[n;H0;D2;+0:12]:[c;...
null
[]
null
null
null
null
4-Amino-5-isobutylamino-10-aza-tricyclo[6.3.1.02,7]dodeca-2(7),3,5-triene-10-carboxylic acid tert-butyl ester (250 mg, 0.74 mmol) from Example 29B was dissolved in ethanol (10 mL) and HOAc (2 mL) and treated with 1-ethoxyethylenemalononitrile (118 mg, 0.87 mmol). The reaction proceeded as in Example 28C (18 h) and was ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine.Secondary amine
null
c1ccc2c(c1)C1C[NH]CC2C1
c1nc2cc3c(cc2[nH]1)C1CNCC3C1
c1nc2cc3c(cc2[nH]1)C1CNCC3C1
HO-
C(C)O
null
null
CC(=O)O.CC(C)CNc1cc2c(cc1N)C1CC2CN(C(=O)OC(C)(C)C)C1>C(C)O>Cc1nc2cc3c(cc2n1CC(C)C)C1CC3CN(C(=O)OC(C)(C)C)C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-c1e478105e0c4ecf87f53b24e0cc7cb9
O=C(N1CC2CC(C1)c1cc([N+](=O)[O-])c([N+](=O)[O-])cc12)C(F)(F)F>>Nc1cc2c(cc1N)C1CC2CN(C(=O)C(F)(F)F)C1
[N+](=O)([O-])C1=CC=2C3CN(CC(C2C=C1[N+](=O)[O-])C3)C(C(F)(F)F)=O>>NC1=CC=2C3CN(CC(C2C=C1N)C3)C(C(F)(F)F)=O
O=[N+:1]([O-])[c:2]1[cH:3][c:4]2[c:5]([cH:6][c:7]1[N+:8](=O)[O-])[CH:9]1[CH2:10][CH:11]2[CH2:12][N:13]([C:14](=[O:15])[C:16]([F:17])([F:18])[F:19])[CH2:20]1>>[NH2:1][c:2]1[cH:3][c:4]2[c:5]([cH:6][c:7]1[NH2:8])[CH:9]1[CH2:10][CH:11]2[CH2:12][N:13]([C:14](=[O:15])[C:16]([F:17])([F:18])[F:19])[CH2:20]1
O=C(N1CC2CC(C1)c1cc([N+](=O)[O-])c([N+](=O)[O-])cc12)C(F)(F)F
Nc1cc2c(cc1N)C1CC2CN(C(=O)C(F)(F)F)C1
null
[OH-].[OH-].[Pd+2]
CO
Reduction
OtherReaction
6748a51a25102225412593c5a930e43f5a8904a80803177de025a6f83c59d65e
a303b0dfb15cc6bade463acf71681cf3ba7580b599dfa4d28d8caac83d08cd17
c1ccc2c(c1)C1CNCC2C1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4](-[N+;H0;D3:5](=O)-[O-]):[c:6]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4](-[NH2;D1;+0:5]):[c:6]
null
[]
null
null
null
null
1-(4,5-Dinitro-10-aza-tricyclo[6.3.1.02,7]dodeca-2(7),3,5-trien-10-yl)-2,2,2-trifluoro-ethanone (3.0 g, 8.70 mmol) was hydrogenated in methanol (30 ml) under a hydrogen atmosphere (45 psi, or approximately 3 atmospheres) over Pd(OH)2 (300 mg of 20 wt %/C, 10% wt). After 2.5 hours the reaction was filtered through a Cel...
10.6084/m9.figshare.5104873.v1
null
Nitro group.Nitro group
Primary amine.Primary amine
null
null
c1ccc2c(c1)C1C[NH]CC2C1
Other
[OH-].[OH-].[Pd+2].CO
null
null
O=C(N1CC2CC(C1)c1cc([N+](=O)[O-])c([N+](=O)[O-])cc12)C(F)(F)F>[OH-].[OH-].[Pd+2].CO>Nc1cc2c(cc1N)C1CC2CN(C(=O)C(F)(F)F)C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-c332f48e15544b4e8f7002466853992f
CC(=O)[O-].O=C(N1CC2CC(C1)c1cc([N+](=O)[O-])c([N+](=O)[O-])cc12)C(F)(F)F>>O=C(N1CC2CC(C1)c1cc([N+](=O)[O-])c(O)cc12)C(F)(F)F
[N+](=O)([O-])C1=CC=2C3CN(CC(C2C=C1[N+](=O)[O-])C3)C(C(F)(F)F)=O.C(C)(=O)[O-].[K+]>>FC(C(=O)N1CC2C=3C=C(C(=CC3C(C1)C2)O)[N+](=O)[O-])(F)F
CC(=O)[O-:16].O=[N+]([O-])[c:15]1[c:11]([N+:12](=[O:13])[O-:14])[cH:10][c:9]2[c:18]([cH:17]1)[CH:5]1[CH2:4][N:3]([C:2](=[O:1])[C:19]([F:20])([F:21])[F:22])[CH2:8][CH:7]2[CH2:6]1>>[O:1]=[C:2]([N:3]1[CH2:4][CH:5]2[CH2:6][CH:7]([CH2:8]1)[c:9]1[cH:10][c:11]([N+:12](=[O:13])[O-:14])[c:15]([OH:16])[cH:17][c:18]12)[C:19]([F:2...
CC(=O)[O-].O=C(N1CC2CC(C1)c1cc([N+](=O)[O-])c([N+](=O)[O-])cc12)C(F)(F)F
O=C(N1CC2CC(C1)c1cc([N+](=O)[O-])c(O)cc12)C(F)(F)F
null
null
CS(=O)C.O
Heteroatom Alkylation and Arylation
OtherReaction
006287576b799c453e649b85a24fa56aa8126d7384c5d3e4e61e59299fcb8c72
86a548d176249a485272aef686188652b058190b5b30134e7b55d29d9f8bbe51
c1ccc2c(c1)C1CNCC2C1
C-C(=O)-[O-;H0;D1:1].O=[N+](-[O-])-[c;H0;D3;+0:2](:[c:3]:[c:4]):[c:5](-[#7;+:6]):[c:7]>>[#7;+:6]-[c:5](:[c:7]):[c;H0;D3;+0:2](-[OH;D1;+0:1]):[c:3]:[c:4]
70
[{"value": 70.0, "product": "FC(C(=O)N1CC2C=3C=C(C(=CC3C(C1)C2)O)[N+](=O)[O-])(F)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 69.7, "product": "FC(C(=O)N1CC2C=3C=C(C(=CC3C(C1)C2)O)[N+](=O)[O-])(F)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
16
HOUR
1-(4,5-Dinitro-10-aza-tricyclo[6.3.1.02,7]dodeca-2(7),3,5-trien-10-yl)-2,2,2-trifluoro-ethanone (900 mg, 2.61 mmol) and potassium acetate (KOAc) (2.6 g, 26.1 mmol) were dissolved in DMSO (10 mL) and warmed with stirring to 100° C. for 16 hours. The mixture was cooled and diluted with H2O (50 mL) then extracted with 80%...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Aromatic alcohol
c1ccc2c(c1)C1C[NH]CC2C1
c1ccc2c(c1)C1C[NH]CC2C1
c1ccc2c(c1)C1C[NH]CC2C1
HO-
CS(=O)C.O
100
16
CC(=O)[O-].O=C(N1CC2CC(C1)c1cc([N+](=O)[O-])c([N+](=O)[O-])cc12)C(F)(F)F>CS(=O)C.O>O=C(N1CC2CC(C1)c1cc([N+](=O)[O-])c(O)cc12)C(F)(F)F
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-64bd259c84b24a4d881ac13f3981aa61
O=C(N1CC2CC(C1)c1cc([N+](=O)[O-])c(O)cc12)C(F)(F)F>>Nc1cc2c(cc1O)C1CC2CN(C(=O)C(F)(F)F)C1
FC(C(=O)N1CC2C=3C=C(C(=CC3C(C1)C2)O)[N+](=O)[O-])(F)F>>FC(C(=O)N1CC2C=3C=C(C(=CC3C(C1)C2)O)N)(F)F
O=[N+:1]([O-])[c:2]1[cH:3][c:4]2[c:5]([cH:6][c:7]1[OH:8])[CH:9]1[CH2:10][CH:11]2[CH2:12][N:13]([C:14](=[O:15])[C:16]([F:17])([F:18])[F:19])[CH2:20]1>>[NH2:1][c:2]1[cH:3][c:4]2[c:5]([cH:6][c:7]1[OH:8])[CH:9]1[CH2:10][CH:11]2[CH2:12][N:13]([C:14](=[O:15])[C:16]([F:17])([F:18])[F:19])[CH2:20]1
O=C(N1CC2CC(C1)c1cc([N+](=O)[O-])c(O)cc12)C(F)(F)F
Nc1cc2c(cc1O)C1CC2CN(C(=O)C(F)(F)F)C1
null
[Pd]
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc2c(c1)C1CNCC2C1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
2,2,2-Trifluoro-1-(4-hydroxy-5-nitro-10-aza-tricyclo[6.3.1.02,7]dodeca-2(7),3,5-trien-10-yl)-ethanone (575 mg, 1.82 mmol) was hydrogenated in methanol under a H2 atmosphere at (45 psi, or approximately 3 atmospheres) over 10% Pd/C (80 mg) for 1.5 hours then filtered through a Celite pad and concentrated to white solids...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccc2c(c1)C1C[NH]CC2C1
Other
[Pd].CO
null
null
O=C(N1CC2CC(C1)c1cc([N+](=O)[O-])c(O)cc12)C(F)(F)F>[Pd].CO>Nc1cc2c(cc1O)C1CC2CN(C(=O)C(F)(F)F)C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-a0e1cb1ebb244b41a71131589d967acf
Cl.Nc1ccc2c(c1)C1CC2CN(C(=O)C(F)(F)F)C1>>O=C(N1CC2CC(C1)c1cc(Cl)ccc12)C(F)(F)F
Cl.Cl.NC1=CC=2C3CN(CC(C2C=C1)C3)C(C(F)(F)F)=O.N(=O)[O-].[Na+]>>ClC1=CC=2C3CN(CC(C2C=C1)C3)C(C(F)(F)F)=O
[ClH:12].N[c:11]1[cH:10][c:9]2[c:15]([cH:14][cH:13]1)[CH:5]1[CH2:4][N:3]([C:2](=[O:1])[C:16]([F:17])([F:18])[F:19])[CH2:8][CH:7]2[CH2:6]1>>[O:1]=[C:2]([N:3]1[CH2:4][CH:5]2[CH2:6][CH:7]([CH2:8]1)[c:9]1[cH:10][c:11]([Cl:12])[cH:13][cH:14][c:15]12)[C:16]([F:17])([F:18])[F:19]
Cl.Nc1ccc2c(c1)C1CC2CN(C(=O)C(F)(F)F)C1
O=C(N1CC2CC(C1)c1cc(Cl)ccc12)C(F)(F)F
null
Cl[Cu]
O
Miscellaneous
OtherReaction
2b7041887f1eceb6f9d882edcffad975e8ab2f416f1382973bb9f8b07f7ae752
1129c10513c603d2647e51dd9713063aaf10bd8a364ed275b9b93c32624e3ba4
c1ccc2c(c1)C1CNCC2C1
N-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[ClH;D0;+0:6]>>[Cl;H0;D1;+0:6]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
95
[{"value": 95.0, "product": "ClC1=CC=2C3CN(CC(C2C=C1)C3)C(C(F)(F)F)=O", "details": "PERCENTYIELD", "is_desired": false}]
60
CELSIUS
null
null
1-(4-Amino-10-aza-tricyclo[6.3.1.02,7]dodeca-2(7),3,5-trien-10-yl)-2,2,2-trifluoro-ethanone (460 mg, 1.7 mmol) was dissolved in H2O (2 mL) and concentrated HCl solution(1 mL) then cooled to 0° C. and treated with a solution of sodium nitrite (NaNO2) (275 mg) in H2O (1 mL) dropwise. To the resulting solution was added a...
10.6084/m9.figshare.5104873.v1
null
Primary amine
Aromatic halide
c1ccc2c(c1)C1C[NH]CC2C1
c1ccc2c(c1)C1C[NH]CC2C1
c1ccc2c(c1)C1C[NH]CC2C1
Other
Cl[Cu].O
60
null
Cl.Nc1ccc2c(c1)C1CC2CN(C(=O)C(F)(F)F)C1>Cl[Cu].O>O=C(N1CC2CC(C1)c1cc(Cl)ccc12)C(F)(F)F
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-838100bfc1eb4170bffb41fdeff481cd
O=C(N1CC2CC(C1)c1cc(Cl)ccc12)C(F)(F)F>>Cl.Clc1ccc2c(c1)C1CNCC2C1
ClC1=CC=2C3CN(CC(C2C=C1)C3)C(C(F)(F)F)=O.C(=O)([O-])[O-].[Na+].[Na+]>>Cl.ClC1=CC=2C3CNCC(C2C=C1)C3
O=C(C(F)(F)F)[N:11]1[CH2:10][CH:9]2[c:7]3[c:6]([cH:5][cH:4][c:3]([Cl:1])[cH:8]3)[CH:13]([CH2:12]1)[CH2:14]2>>[ClH:1].[Cl:2][c:3]1[cH:4][cH:5][c:6]2[c:7]([cH:8]1)[CH:9]1[CH2:10][NH:11][CH2:12][CH:13]2[CH2:14]1
O=C(N1CC2CC(C1)c1cc(Cl)ccc12)C(F)(F)F
Cl.Clc1ccc2c(c1)C1CNCC2C1
null
null
CO.O
Miscellaneous
Hydrogenolysis of tertiary amines
a6137ef918539e263903a8a4ae0ea118fd5c2cd29e3061a4891158b906dcc255
c917f007c6daf2ba5ac5faecc6c9acfa67f53d875fa50728fec5dcddec33c9e4
c1ccc2c(c1)C1CNCC2C1
F-C(-F)(-F)-C(=O)-[N;H0;D3;+0:1](-[C:2]-[C:3]-[c:4]:[c:5]:[c;H0;D3;+0:6](-[Cl;H0;D1;+0:7]):[c:8]:[c:9])-[C:10]-[C:11]>>[C:11]-[C:10]-[NH;D2;+0:1]-[C:2]-[C:3]-[c:4]:[c:5]:[c;H0;D3;+0:6](-[Cl;D1;H0:12]):[c:8]:[c:9].[ClH;D0;+0:7]
null
[]
null
null
2
HOUR
1-(4-Chloro-10-aza-tricyclo[6.3.1.02,7]dodeca-2(7),3,5-trien-10-yl)-2,2,2-trifluoro-ethanone (470 mg, 1.62 mmol) and Na2CO3 (344 mg, 3.24 mmol) in methanol (30 mL) and H2O (10 mL) were heated to reflux. After 2 hours, the reaction was cooled and diluted with water then extracted with ethyl acetate (4×40 mL), dried (Na2...
10.6084/m9.figshare.5104873.v1
null
Trifluoro group.Aromatic halide.Tertiary amide
Aromatic halide.Secondary amine
c1ccc2c(c1)C1C[NH]CC2C1
c1ccc2c(c1)C1CNCC2C1
c1ccc2c(c1)C1CNCC2C1
Other
CO.O
null
2
O=C(N1CC2CC(C1)c1cc(Cl)ccc12)C(F)(F)F>CO.O>Cl.Clc1ccc2c(c1)C1CNCC2C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-61f22df1abf941a0bb796b93e209b430
Nc1ccc2c(c1)C1CC2CN(C(=O)C(F)(F)F)C1.[I-]>>O=C(N1CC2CC(C1)c1cc(I)ccc12)C(F)(F)F
[I-].[K+].NC1=CC=2C3CN(CC(C2C=C1)C3)C(C(F)(F)F)=O.N(=O)[O-].[Na+]>>IC1=CC=2C3CN(CC(C2C=C1)C3)C(C(F)(F)F)=O
N[c:11]1[cH:10][c:9]2[c:15]([cH:14][cH:13]1)[CH:5]1[CH2:4][N:3]([C:2](=[O:1])[C:16]([F:17])([F:18])[F:19])[CH2:8][CH:7]2[CH2:6]1.[I-:12]>>[O:1]=[C:2]([N:3]1[CH2:4][CH:5]2[CH2:6][CH:7]([CH2:8]1)[c:9]1[cH:10][c:11]([I:12])[cH:13][cH:14][c:15]12)[C:16]([F:17])([F:18])[F:19]
Nc1ccc2c(c1)C1CC2CN(C(=O)C(F)(F)F)C1.[I-]
O=C(N1CC2CC(C1)c1cc(I)ccc12)C(F)(F)F
null
null
O.OS(=O)(=O)O
Functional Group Interconversion
OtherReaction
d85248fa2dcf066a404d25d0a3dc9531961e235579e6a0103df5b0ec1c500653
9c224743a26d9e1c3135e4817dd611aec414d8ea156f02200a3aef865be78b01
c1ccc2c(c1)C1CNCC2C1
N-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[I-;H0;D0:6]>>[I;H0;D1;+0:6]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
null
[]
null
null
18
HOUR
1-(4-Amino-10-aza-tricyclo[6.3.1.02,7]dodeca-2(7),3,5-trien-10-yl)-2,2,2-trifluoro-ethanone (500 mg, 1.85 mmol) was dissolved in H2O (5 mL) and concentrated H2SO4 solution (0.5 mL) then cooled to 0° C. and treated with a solution of sodium nitrite (NaNO2) (140 mg, 2.04 mmol) in H2O (2 mL) dropwise. Potassium iodide (46...
10.6084/m9.figshare.5104873.v1
null
Primary amine
Aromatic halide
c1ccc2c(c1)C1C[NH]CC2C1
c1ccc2c(c1)C1C[NH]CC2C1
c1ccc2c(c1)C1C[NH]CC2C1
Other
O.OS(=O)(=O)O
null
18
Nc1ccc2c(c1)C1CC2CN(C(=O)C(F)(F)F)C1.[I-]>O.OS(=O)(=O)O>O=C(N1CC2CC(C1)c1cc(I)ccc12)C(F)(F)F
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-6a5a32196acf4e768cde31de4aed7d60
CC(C)(C)OC(=O)N1CC2CC(C1)c1cc(C#N)ccc12>>N#Cc1ccc2c(c1)C1CNCC2C1
C(C)(C)(C)OC(=O)N1CC2C=3C=CC(=CC3C(C1)C2)C#N.C(C)(=O)OCC.Cl>>Cl.C12C=3C=C(C=CC3C(CNC1)C2)C#N
CC(C)(C)OC(=O)[N:12]1[CH2:11][CH:10]2[c:8]3[c:7]([cH:6][cH:5][c:4]([C:3]#[N:2])[cH:9]3)[CH:14]([CH2:13]1)[CH2:15]2>>[N:2]#[C:3][c:4]1[cH:5][cH:6][c:7]2[c:8]([cH:9]1)[CH:10]1[CH2:11][NH:12][CH2:13][CH:14]2[CH2:15]1
CC(C)(C)OC(=O)N1CC2CC(C1)c1cc(C#N)ccc12
N#Cc1ccc2c(c1)C1CNCC2C1
null
null
null
Reduction
Boc amine deprotection
16a87a91f73ba41dd2fbaeff5b0b018f397c5ad5c549cbd7af59e94acd9700c1
a94b29c7264c852156fc1cdd4a0951a4fc26c06d0edc9e50c743825dbf79e3fd
c1ccc2c(c1)C1CNCC2C1
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1](-[C:2]-[C:3])-[C:4]-[C:5]>>[C:3]-[C:2]-[NH;D2;+0:1]-[C:4]-[C:5]
null
[]
null
null
18
HOUR
4-Cyano-10-aza-tricyclo[6.3.1.02,7]dodeca-2(7),3,5-triene-10-carboxylic acid tert-butyl ester was treated with 3N HCl ethyl acetate (6 mL) and warmed to reflux for 2 hours, then concentrated, dissolved in a minimum of methanol which was saturated with Et2O and stirred 18 hours. The product was collected by filtration (...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Secondary amine
c1ccc2c(c1)C1C[NH]CC2C1
c1ccc2c(c1)C1CNCC2C1
c1ccc2c(c1)C1CNCC2C1
HO-
null
null
18
CC(C)(C)OC(=O)N1CC2CC(C1)c1cc(C#N)ccc12>>N#Cc1ccc2c(c1)C1CNCC2C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-99b5561f14694dee9f68132e67b69d9b
CC(=O)Cl.O=C(N1CC2CC(C1)c1ccccc12)C(F)(F)F>>CC(=O)c1ccc2c(c1)C1CC2CN(C(=O)C(F)(F)F)C1
C(=O)(O)[O-].[Na+].C12C=3C=CC=CC3C(CN(C1)C(C(F)(F)F)=O)C2.C(=O)(C)Cl.[Cl-].[Al+3].[Cl-].[Cl-]>>C(C)(=O)C1=CC=2C3CN(CC(C2C=C1)C3)C(C(F)(F)F)=O
Cl[C:2]([CH3:1])=[O:3].[cH:4]1[cH:5][cH:6][c:7]2[c:8]([cH:9]1)[CH:10]1[CH2:11][CH:12]2[CH2:13][N:14]([C:15](=[O:16])[C:17]([F:18])([F:19])[F:20])[CH2:21]1>>[CH3:1][C:2](=[O:3])[c:4]1[cH:5][cH:6][c:7]2[c:8]([cH:9]1)[CH:10]1[CH2:11][CH:12]2[CH2:13][N:14]([C:15](=[O:16])[C:17]([F:18])([F:19])[F:20])[CH2:21]1
CC(=O)Cl.O=C(N1CC2CC(C1)c1ccccc12)C(F)(F)F
CC(=O)c1ccc2c(c1)C1CC2CN(C(=O)C(F)(F)F)C1
null
null
ClCCCl
C-C Coupling
Friedel-Crafts acylation
440542c1d377bda35f0172763cc622606266c84265c45cd45a3812b0fb5cd1dc
fe2a4a0dfbb5b71b9a065e092364c64b22b4eb1ad4d6ba2a1e8edc9d31fce3e4
c1ccc2c(c1)C1CNCC2C1
Cl-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[c:4]:[c:5]:[cH;D2;+0:6]:[c:7]:[c:8]>>[C;D1;H3:2]-[C;H0;D3;+0:1](=[O;D1;H0:3])-[c;H0;D3;+0:6](:[c:5]:[c:4]):[c:7]:[c:8]
null
[]
null
null
30
MINUTE
1-(10-Aza-tricyclo[6.3.1.02,7]dodeca-2(7),3,5-trien-10-yl)-2,2,2-trifluoro-ethanone (253 mg, 1.0 mmol) and AcCl (0.68 mL, 10 mmol) were dissolved in DCE (3 mL) and treated with aluminum chloride (AlCl3) (667 mg, 5.0 mmol). The resulting yellow mixture was stirred for 30 minutes then poured over ice and saturated aqueou...
10.6084/m9.figshare.5104873.v1
null
Acyl halide
Ketone
c1ccc2c(c1)C1C[NH]CC2C1
c1ccc2c(c1)C1C[NH]CC2C1
c1ccc2c(c1)C1C[NH]CC2C1
HCl
ClCCCl
null
0.5
CC(=O)Cl.O=C(N1CC2CC(C1)c1ccccc12)C(F)(F)F>ClCCCl>CC(=O)c1ccc2c(c1)C1CC2CN(C(=O)C(F)(F)F)C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-b60e3c5ebb754101980b3f930fd4d1c7
CC(=O)c1ccc2c(c1)C1CC2CN(C(=O)OC(C)(C)C)C1>>CC(=O)c1ccc2c(c1)C1CNCC2C1
C(C)(C)(C)OC(=O)N1CC2C=3C=CC(=CC3C(C1)C2)C(C)=O.C(C)(=O)OCC.Cl>>Cl.C12C=3C=C(C=CC3C(CNC1)C2)C(C)=O
CC(C)(C)OC(=O)[N:12]1[CH2:11][CH:10]2[c:8]3[c:7]([cH:6][cH:5][c:4]([C:2]([CH3:1])=[O:3])[cH:9]3)[CH:14]([CH2:13]1)[CH2:15]2>>[CH3:1][C:2](=[O:3])[c:4]1[cH:5][cH:6][c:7]2[c:8]([cH:9]1)[CH:10]1[CH2:11][NH:12][CH2:13][CH:14]2[CH2:15]1
CC(=O)c1ccc2c(c1)C1CC2CN(C(=O)OC(C)(C)C)C1
CC(=O)c1ccc2c(c1)C1CNCC2C1
null
null
null
Reduction
Boc amine deprotection
16a87a91f73ba41dd2fbaeff5b0b018f397c5ad5c549cbd7af59e94acd9700c1
a94b29c7264c852156fc1cdd4a0951a4fc26c06d0edc9e50c743825dbf79e3fd
c1ccc2c(c1)C1CNCC2C1
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1](-[C:2]-[C:3])-[C:4]-[C:5]>>[C:3]-[C:2]-[NH;D2;+0:1]-[C:4]-[C:5]
null
[]
70
CELSIUS
null
null
4-Acetyl-10-aza-tricyclo[6.3.1.02,7]dodeca-2(7),3,5-triene-10-carboxylic acid tert-butyl ester (190 mg, 0.63 mmol) was treated with excess 3N HCl ethyl acetate and warmed to 70° C. for 1 hour then concentrated and dissolved in a minimum of methanol. The resulting solution was saturated with Et2O and stirred. After 18 h...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Secondary amine
c1ccc2c(c1)C1C[NH]CC2C1
c1ccc2c(c1)C1CNCC2C1
c1ccc2c(c1)C1CNCC2C1
HO-
null
70
null
CC(=O)c1ccc2c(c1)C1CC2CN(C(=O)OC(C)(C)C)C1>>CC(=O)c1ccc2c(c1)C1CNCC2C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-b1f2c8cc27034c179f1b4822f27ad1dc
CC(=O)Oc1ccc2c(c1)C1CC2CN(C(=O)C(F)(F)F)C1>>O=C(N1CC2CC(C1)c1cc(O)ccc12)C(F)(F)F
FC(C(=O)N1CC2C=3C=CC(=CC3C(C1)C2)OC(C)=O)(F)F.C(=O)(O)[O-].[Na+]>>FC(C(=O)N1CC2C=3C=CC(=CC3C(C1)C2)O)(F)F
CC(=O)[O:12][c:11]1[cH:10][c:9]2[c:15]([cH:14][cH:13]1)[CH:5]1[CH2:4][N:3]([C:2](=[O:1])[C:16]([F:17])([F:18])[F:19])[CH2:8][CH:7]2[CH2:6]1>>[O:1]=[C:2]([N:3]1[CH2:4][CH:5]2[CH2:6][CH:7]([CH2:8]1)[c:9]1[cH:10][c:11]([OH:12])[cH:13][cH:14][c:15]12)[C:16]([F:17])([F:18])[F:19]
CC(=O)Oc1ccc2c(c1)C1CC2CN(C(=O)C(F)(F)F)C1
O=C(N1CC2CC(C1)c1cc(O)ccc12)C(F)(F)F
null
null
CO
Reduction
Hydrolysis or Hydrogenolysis of Carboxylic Esters or Thioesters
db7d50f1ad65e3456617ab9bc6ab5b9ede0e069a6dd971d117a653e2a40b05de
efe1c37482b229370967d04d1a68db10ee663983a92b84fa0f009f5bb178597f
c1ccc2c(c1)C1CNCC2C1
C-C(=O)-[O;H0;D2;+0:1]-[c:2](:[c:3]):[c:4]>>[OH;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
Acetic acid 10-trifluoroacetyl-10-aza-tricyclo[6.3.1.02,7]dodeca-2(7),3,5-trien-4-yl ester (900 mg, 2.87 mmol) was stirred in methanol (20 mL) and saturated aqueous NaHCO3 solution (15 mL) for 48 hours. The mixture was concentrated, diluted with H2O and extracted with CH2Cl2 (3×20 mL) then dried through a cotton plug. ...
10.6084/m9.figshare.5104873.v1
null
Ester
Aromatic alcohol
null
null
c1ccc2c(c1)C1C[NH]CC2C1
HO-
CO
null
null
CC(=O)Oc1ccc2c(c1)C1CC2CN(C(=O)C(F)(F)F)C1>CO>O=C(N1CC2CC(C1)c1cc(O)ccc12)C(F)(F)F
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-bca363c09c8445f68bf4196a6fca5bb7
O=C(N1CC2CC(C1)c1cc(O)ccc12)C(F)(F)F>>Oc1ccc2c(c1)C1CNCC2C1
FC(C(=O)N1CC2C=3C=CC(=CC3C(C1)C2)O)(F)F.C(=O)([O-])[O-].[Na+].[Na+].C(C)(=O)OCC.Cl>>Cl.C12C=3C=C(C=CC3C(CNC1)C2)O
O=C(C(F)(F)F)[N:11]1[CH2:10][CH:9]2[c:7]3[c:6]([cH:5][cH:4][c:3]([OH:2])[cH:8]3)[CH:13]([CH2:12]1)[CH2:14]2>>[OH:2][c:3]1[cH:4][cH:5][c:6]2[c:7]([cH:8]1)[CH:9]1[CH2:10][NH:11][CH2:12][CH:13]2[CH2:14]1
O=C(N1CC2CC(C1)c1cc(O)ccc12)C(F)(F)F
Oc1ccc2c(c1)C1CNCC2C1
null
null
CO.O
Reduction
Hydrogenolysis of tertiary amines
f46cbee729057ebd415120d06c8d35552e9f6cc6e71a027737f358de057e1ec8
9d0759623d33e2d41aafe1af3bb1025d4d7a88f20060c872279b889c110cab65
c1ccc2c(c1)C1CNCC2C1
F-C(-F)(-F)-C(=O)-[N;H0;D3;+0:1](-[C:2]-[C:3])-[C:4]-[C:5]>>[C:5]-[C:4]-[NH;D2;+0:1]-[C:2]-[C:3]
null
[]
65
CELSIUS
null
null
2,2,2-Trifluoro-1-(4-hydroxy-10-aza-tricyclo[6.3.1.02,7]dodeca-2(7),3,5-trien-10-yl)-ethanone (50 mg, 0.184 mmol) was dissolved in methanol/H2O (3/1, 5 mL), treated with Na2CO3(s) (40 mg, 0.369 mmol) and warmed to 65° C. for 2 hours. The mixture was concentrated, diluted with H2O and extracted with CH2Cl2 (3×20 mL) the...
10.6084/m9.figshare.5104873.v1
null
Trifluoro group.Tertiary amide
Secondary amine
c1ccc2c(c1)C1C[NH]CC2C1
c1ccc2c(c1)C1CNCC2C1
c1ccc2c(c1)C1CNCC2C1
Other
CO.O
65
null
O=C(N1CC2CC(C1)c1cc(O)ccc12)C(F)(F)F>CO.O>Oc1ccc2c(c1)C1CNCC2C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-35ab5842722f47c4979b47f623f112e4
CC(=O)c1cc2c(cc1O)C1CC2CN(C(=O)C(F)(F)F)C1.NO>>CC(=NO)c1cc2c(cc1O)C1CC2CN(C(=O)C(F)(F)F)C1
C(C)(=O)C1=CC=2C3CN(CC(C2C=C1O)C3)C(C(F)(F)F)=O.Cl.NO.C(C)(=O)[O-].[Na+]>>FC(C(=O)N1CC2C=3C=C(C(=CC3C(C1)C2)O)C(C)=NO)(F)F
O=[C:2]([CH3:1])[c:5]1[cH:6][c:7]2[c:8]([cH:9][c:10]1[OH:11])[CH:12]1[CH2:13][CH:14]2[CH2:15][N:16]([C:17](=[O:18])[C:19]([F:20])([F:21])[F:22])[CH2:23]1.[NH2:3][OH:4]>>[CH3:1][C:2](=[N:3][OH:4])[c:5]1[cH:6][c:7]2[c:8]([cH:9][c:10]1[OH:11])[CH:12]1[CH2:13][CH:14]2[CH2:15][N:16]([C:17](=[O:18])[C:19]([F:20])([F:21])[F:2...
CC(=O)c1cc2c(cc1O)C1CC2CN(C(=O)C(F)(F)F)C1.NO
CC(=NO)c1cc2c(cc1O)C1CC2CN(C(=O)C(F)(F)F)C1
null
null
CO.O
Heteroatom Alkylation and Arylation
OtherReaction
b5fd91d879f097d0ef2e8e2d3ef7d2ef0195968870a9602a47b8324c601790b9
1a0ef15294bdb221fb8888b5d4c7fcf00473b11e53da288791d32747daa48d23
c1ccc2c(c1)C1CNCC2C1
O=[C;H0;D3;+0:1](-[C;D1;H3:2])-[c:3](:[c:4]):[c:5].[NH2;D1;+0:6]-[O;D1;H1:7]>>[C;D1;H3:2]-[C;H0;D3;+0:1](=[N;H0;D2;+0:6]-[O;D1;H1:7])-[c:3](:[c:4]):[c:5]
93
[{"value": 93.0, "product": "FC(C(=O)N1CC2C=3C=C(C(=CC3C(C1)C2)O)C(C)=NO)(F)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 89.1, "product": "FC(C(=O)N1CC2C=3C=C(C(=CC3C(C1)C2)O)C(C)=NO)(F)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
1-(4-Acetyl-5-hydroxy-10-aza-tricyclo[6.3.1.02,7]dodeca-2(7),3,5-trien-10-yl)-2,2,2-trifluoro-ethanone (190 mg, 0.605 mmol), hydroxylamine HCl (99 mg, 1.21 mmol) and sodium acetate (118 mg, 1.21 mmol) were combined in methanol (4 mL) and H2O (1 mL) and warmed to 65° C. for 18 hours. The mixture was cooled, diluted with...
10.6084/m9.figshare.5104873.v1
null
Ketone.Primary amine
Oxime
null
null
c1ccc2c(c1)C1C[NH]CC2C1
HO-
CO.O
null
null
CC(=O)c1cc2c(cc1O)C1CC2CN(C(=O)C(F)(F)F)C1.NO>CO.O>CC(=NO)c1cc2c(cc1O)C1CC2CN(C(=O)C(F)(F)F)C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-032980fbd7fc499094c1d87313b64b51
O=C(N1CC2CC(C1)c1ccccc12)C(F)(F)F.O=S(=O)(O)Cl>>O=C(N1CC2CC(C1)c1cc(S(=O)(=O)Cl)ccc12)C(F)(F)F
C12C=3C=CC=CC3C(CN(C1)C(C(F)(F)F)=O)C2.ClS(=O)(=O)O>>FC(C(=O)N1CC2C=3C=CC(=CC3C(C1)C2)S(=O)(=O)Cl)(F)F
[O:1]=[C:2]([N:3]1[CH2:4][CH:5]2[CH2:6][CH:7]([CH2:8]1)[c:9]1[cH:10][cH:11][cH:16][cH:17][c:18]12)[C:19]([F:20])([F:21])[F:22].O=[S:12]([OH:13])(=[O:14])[Cl:15]>>[O:1]=[C:2]([N:3]1[CH2:4][CH:5]2[CH2:6][CH:7]([CH2:8]1)[c:9]1[cH:10][c:11]([S:12](=[O:13])(=[O:14])[Cl:15])[cH:16][cH:17][c:18]12)[C:19]([F:20])([F:21])[F:22]
O=C(N1CC2CC(C1)c1ccccc12)C(F)(F)F.O=S(=O)(O)Cl
O=C(N1CC2CC(C1)c1cc(S(=O)(=O)Cl)ccc12)C(F)(F)F
null
null
null
Protection
Aromatic sulfonyl chlorination
e5a1262dd987e1cbc7fec85c9059213cf3049113a4cf5e7238533ed51231b9db
c731d053565135be022f3edbe36cf28a9b4364ca579bdb183b2db9578bab4695
c1ccc2c(c1)C1CNCC2C1
O=[S;H0;D4;+0:1](-[Cl;D1;H0:2])(=[O;D1;H0:3])-[OH;D1;+0:4].[c:5]:[c:6]:[cH;D2;+0:7]:[c:8]:[c:9]>>[Cl;D1;H0:2]-[S;H0;D4;+0:1](=[O;D1;H0:3])(=[O;H0;D1;+0:4])-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:6]:[c:5]
87
[{"value": 87.0, "product": "FC(C(=O)N1CC2C=3C=CC(=CC3C(C1)C2)S(=O)(=O)Cl)(F)F", "details": "PERCENTYIELD", "is_desired": false}]
null
null
5
MINUTE
1-(10-Aza-tricyclo[6.3.1.02,7]dodeca-2(7),3,5-trien-10-yl)-2,2,2-trifluoro-ethanone mg, 2.1 mmol) was added to chlorosulfonic acid (2 mL, 30 mmol) and stirred for 5 minutes. The mixture was quenched with ice, extracted with ethyl acetate, dried (Na2SO4), filtered and concentrated to provide an oil (640 mg, 87%). (TLC 3...
10.6084/m9.figshare.5104873.v1
null
null
Sulfonyl halide
c1ccc2c(c1)C1C[NH]CC2C1
c1ccc2c(c1)C1C[NH]CC2C1
c1ccc2c(c1)C1C[NH]CC2C1
HO-
null
null
0.083333
O=C(N1CC2CC(C1)c1ccccc12)C(F)(F)F.O=S(=O)(O)Cl>>O=C(N1CC2CC(C1)c1cc(S(=O)(=O)Cl)ccc12)C(F)(F)F
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-88a46a881e0040319b6f874fdc35cd86
Nc1cc2c(cc1O)C1CC2CN(C(=O)C(F)(F)F)C1.O=C(Cl)Cc1ccccc1>>Cl.c1ccc(Cc2nc3cc4c(cc3o2)C2CNCC4C2)cc1
FC(C(=O)N1CC2C=3C=C(C(=CC3C(C1)C2)O)N)(F)F.C1(=CC=CC=C1)CC(=O)Cl>>Cl.C(C1=CC=CC=C1)C=1OC2=CC=3C4CNCC(C3C=C2N1)C4
O=C(C(F)(F)F)[N:18]1[CH2:17][CH:16]2[c:12]3[c:11]([cH:10][c:9]([NH2:8])[c:14]([OH:15])[cH:13]3)[CH:20]([CH2:19]1)[CH2:21]2.O=[C:7]([Cl:1])[CH2:6][c:5]1[cH:4][cH:3][cH:2][cH:23][cH:22]1>>[ClH:1].[cH:2]1[cH:3][cH:4][c:5]([CH2:6][c:7]2[n:8][c:9]3[cH:10][c:11]4[c:12]([cH:13][c:14]3[o:15]2)[CH:16]2[CH2:17][NH:18][CH2:19][CH...
Nc1cc2c(cc1O)C1CC2CN(C(=O)C(F)(F)F)C1.O=C(Cl)Cc1ccccc1
Cl.c1ccc(Cc2nc3cc4c(cc3o2)C2CNCC4C2)cc1
null
null
null
Aromatic Heterocycle Formation
OtherReaction
195dcfd9849a6bacc638b00f2ff33e90dc043dfa52207d61d6fb173e8f01110b
17d0c0b2e2a3248b62a86941fc178c06b92c2384911e7d108e6679cac538949f
c1ccc(Cc2nc3cc4c(cc3o2)C2CNCC4C2)cc1
F-C(-F)(-F)-C(=O)-[N;H0;D3;+0:1](-[C:2]-[C:3])-[C:4]-[C:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9](-[OH;D1;+0:10]):[c:11].O=[C;H0;D3;+0:12](-[Cl;H0;D1;+0:13])-[C:14]-[c:15]>>[C:3]-[C:2]-[NH;D2;+0:1]-[C:4]-[C:5].[c:8]:[c:7]1:[n;H0;D2;+0:6]:[c;H0;D3;+0:12](-[C:14]-[c:15]):[o;H0;D2;+0:10]:[c:9]:1:[c:11].[ClH;D0;+0:13]
null
[]
null
null
null
null
2,2,2-Trifluoro-1-(4-hydroxy-5-amino-10-aza-tricyclo[6.3.1.02,7]dodeca-2(7),3,5-trien-10-yl)-ethanone and phenyl-acetyl chloride were converted to the title compound following the procedures described in Example 54. 1H NMR (400 MHz, CD3OD) δ 7.63 (s, 1H), 7.58 (s, 1H), 7.36–7.24 (5H), 4.29 (s, 2H), 3.46 (d, J=2.5 Hz, 2...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Trifluoro group.Tertiary amide.Aromatic alcohol.Primary amine
Secondary amine
c1ccc2c(c1)C1C[NH]CC2C1
c1nc2cc3c(cc2o1)C1CNCC3C1
c1ccccc1.c1nc2cc3c(cc2o1)C1CNCC3C1
HF
null
null
null
Nc1cc2c(cc1O)C1CC2CN(C(=O)C(F)(F)F)C1.O=C(Cl)Cc1ccccc1>>Cl.c1ccc(Cc2nc3cc4c(cc3o2)C2CNCC4C2)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-128b4aeccb114b75ba2665b33ee49ad6
CCC(=O)Cl.Nc1cc2c(cc1O)C1CC2CN(C(=O)C(F)(F)F)C1>>CCc1nc2cc3c(cc2o1)C1CNCC3C1.Cl
FC(C(=O)N1CC2C=3C=C(C(=CC3C(C1)C2)O)N)(F)F.C(CC)(=O)Cl>>Cl.C(C)C=1OC2=CC=3C4CNCC(C3C=C2N1)C4
O=[C:3]([CH2:2][CH3:1])[Cl:18].O=C(C(F)(F)F)[N:14]1[CH2:13][CH:12]2[c:8]3[c:7]([cH:6][c:5]([NH2:4])[c:10]([OH:11])[cH:9]3)[CH:16]([CH2:15]1)[CH2:17]2>>[CH3:1][CH2:2][c:3]1[n:4][c:5]2[cH:6][c:7]3[c:8]([cH:9][c:10]2[o:11]1)[CH:12]1[CH2:13][NH:14][CH2:15][CH:16]3[CH2:17]1.[ClH:18]
CCC(=O)Cl.Nc1cc2c(cc1O)C1CC2CN(C(=O)C(F)(F)F)C1
CCc1nc2cc3c(cc2o1)C1CNCC3C1.Cl
null
null
null
Aromatic Heterocycle Formation
OtherReaction
195dcfd9849a6bacc638b00f2ff33e90dc043dfa52207d61d6fb173e8f01110b
17d0c0b2e2a3248b62a86941fc178c06b92c2384911e7d108e6679cac538949f
c1nc2cc3c(cc2o1)C1CNCC3C1
F-C(-F)(-F)-C(=O)-[N;H0;D3;+0:1](-[C:2]-[C:3])-[C:4]-[C:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9](-[OH;D1;+0:10]):[c:11].O=[C;H0;D3;+0:12](-[Cl;H0;D1;+0:13])-[C:14]-[C;D1;H3:15]>>[C;D1;H3:15]-[C:14]-[c;H0;D3;+0:12]1:[n;H0;D2;+0:6]:[c:7](:[c:8]):[c:9](:[c:11]):[o;H0;D2;+0:10]:1.[C:3]-[C:2]-[NH;D2;+0:1]-[C:4]-[C:5].[ClH;D0;+0...
null
[]
null
null
null
null
2,2,2-Trifluoro-1-(4-hydroxy-5-amino-10-aza-tricyclo[6.3.1.02,7]dodeca-2(7),3,5-trien-10-yl)-ethanone and propionyl chloride were converted to the title compound following the procedures described in Example 40 and Goldstein, S. W.; Dambek, P. J. J. Het. Chem. 1990, 27, 335. 1H NMR (400 MHz, CD3OD) δ 7.64 (s, 1H), 7.62...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Trifluoro group.Tertiary amide.Aromatic alcohol.Primary amine
Secondary amine
c1ccc2c(c1)C1C[NH]CC2C1
c1nc2cc3c(cc2o1)C1CNCC3C1
c1nc2cc3c(cc2o1)C1CNCC3C1
HF
null
null
null
CCC(=O)Cl.Nc1cc2c(cc1O)C1CC2CN(C(=O)C(F)(F)F)C1>>CCc1nc2cc3c(cc2o1)C1CNCC3C1.Cl
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-ddf33257574b40a69f6d86c33b8b371a
CC(C)C(=O)Cl.Nc1cc2c(cc1O)C1CC2CN(C(=O)C(F)(F)F)C1>>CC(C)c1nc2cc3c(cc2o1)C1CNCC3C1.Cl
FC(C(=O)N1CC2C=3C=C(C(=CC3C(C1)C2)O)N)(F)F.C(C(C)C)(=O)Cl>>Cl.C(C)(C)C=1OC2=CC=3C4CNCC(C3C=C2N1)C4
O=[C:4]([CH:2]([CH3:1])[CH3:3])[Cl:19].O=C(C(F)(F)F)[N:15]1[CH2:14][CH:13]2[c:9]3[c:8]([cH:7][c:6]([NH2:5])[c:11]([OH:12])[cH:10]3)[CH:17]([CH2:16]1)[CH2:18]2>>[CH3:1][CH:2]([CH3:3])[c:4]1[n:5][c:6]2[cH:7][c:8]3[c:9]([cH:10][c:11]2[o:12]1)[CH:13]1[CH2:14][NH:15][CH2:16][CH:17]3[CH2:18]1.[ClH:19]
CC(C)C(=O)Cl.Nc1cc2c(cc1O)C1CC2CN(C(=O)C(F)(F)F)C1
CC(C)c1nc2cc3c(cc2o1)C1CNCC3C1.Cl
null
null
null
Aromatic Heterocycle Formation
OtherReaction
195dcfd9849a6bacc638b00f2ff33e90dc043dfa52207d61d6fb173e8f01110b
17d0c0b2e2a3248b62a86941fc178c06b92c2384911e7d108e6679cac538949f
c1nc2cc3c(cc2o1)C1CNCC3C1
F-C(-F)(-F)-C(=O)-[N;H0;D3;+0:1](-[C:2]-[C:3])-[C:4]-[C:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9](-[OH;D1;+0:10]):[c:11].O=[C;H0;D3;+0:12](-[Cl;H0;D1;+0:13])-[C:14](-[C;D1;H3:15])-[C;D1;H3:16]>>[C;D1;H3:15]-[C:14](-[C;D1;H3:16])-[c;H0;D3;+0:12]1:[n;H0;D2;+0:6]:[c:7](:[c:8]):[c:9](:[c:11]):[o;H0;D2;+0:10]:1.[C:3]-[C:2]-[NH;D...
null
[]
null
null
null
null
2,2,2-Trifluoro-1-(4-hydroxy-5-amino-10-aza-tricyclo[6.3.1.02,7]dodeca-2(7),3,5-trien-10-yl)-ethanone and isobutyryl chloride were converted to the title compound following the procedures described in Example 54. (TLC 25% ethyl acetate/hexanes Rf 0.14). 1H NMR (400 MHz, CD3OD) δ 7.65 (2H), 3.49 (br s, 2H), 3.41 (d, J=1...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Trifluoro group.Tertiary amide.Aromatic alcohol.Primary amine
Secondary amine
c1ccc2c(c1)C1C[NH]CC2C1
c1nc2cc3c(cc2o1)C1CNCC3C1
c1nc2cc3c(cc2o1)C1CNCC3C1
HF
null
null
null
CC(C)C(=O)Cl.Nc1cc2c(cc1O)C1CC2CN(C(=O)C(F)(F)F)C1>>CC(C)c1nc2cc3c(cc2o1)C1CNCC3C1.Cl
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-1760007316da4df791d25f5e9c52543d
COC(=O)CC(OC)OC>>COC(CC(=O)[O-])OC.[Li+]
COC(CC(OC)OC)=O.O[Li].O.O>>[Li+].COC(CC(=O)[O-])OC
C[O:7][C:5]([CH2:4][CH:3]([O:2][CH3:1])[O:8][CH3:9])=[O:6]>>[CH3:1][O:2][CH:3]([CH2:4][C:5](=[O:6])[O-:7])[O:8][CH3:9].[Li+:10]
COC(=O)CC(OC)OC
COC(CC(=O)[O-])OC.[Li+]
null
null
C1CCOC1
Functional Group Interconversion
Ester to carboxylate
821210f6f99f2510a1cab460144f356df713620aaf5f176ae325aca686567da7
5e32b8721010c33cc6df2b6213aa79bfd72016baf9e10bd582a623b626f4f641
null
C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](-[O-;H0;D1:1])=[O;D1;H0:4]
98.7
[{"value": 98.7, "product": "[Li+].COC(CC(=O)[O-])OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
(Related to methods described in Alabaster, C. T. et. al., J. Med. Chem. 1988, 31, 2048–2056.) 3,3-Dimethoxypropanoic acid methyl ester (14.25 g, 96.2 mmol) in THF (100 mL) was treated with LiOH.H2O (2.5 g, 106 mmol) and H2O (2 mL). The mixture was brought to reflux for 4 hours, cooled to room temperature and azeotropi...
10.6084/m9.figshare.5104873.v1
null
Ester
null
null
null
null
null
C1CCOC1
null
null
COC(=O)CC(OC)OC>C1CCOC1>COC(CC(=O)[O-])OC.[Li+]
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-b4d6b3277093439c8ceae4c543cc0e02
O=C(c1c2c(cc3[nH]c(=O)ccc13)C1CNCC2C1)C(F)(F)F.O=P(Cl)(Cl)Cl>>O=C(c1c2c(cc3nc(Cl)ccc13)C1CNCC2C1)C(F)(F)F
C12C=3C=C4NC(C=CC4=C(C3C(CNC1)C2)C(C(F)(F)F)=O)=O.O=P(Cl)(Cl)Cl>>ClC1=NC2=CC=3C4CNCC(C3C(=C2C=C1)C(C(F)(F)F)=O)C4
O=[c:9]1[nH:8][c:7]2[cH:6][c:5]3[c:4]([c:3]([C:2](=[O:1])[C:20]([F:21])([F:22])[F:23])[c:13]2[cH:12][cH:11]1)[CH:18]1[CH2:17][NH:16][CH2:15][CH:14]3[CH2:19]1.O=P(Cl)(Cl)[Cl:10]>>[O:1]=[C:2]([c:3]1[c:4]2[c:5]([cH:6][c:7]3[n:8][c:9]([Cl:10])[cH:11][cH:12][c:13]13)[CH:14]1[CH2:15][NH:16][CH2:17][CH:18]2[CH2:19]1)[C:20]([F...
O=C(c1c2c(cc3[nH]c(=O)ccc13)C1CNCC2C1)C(F)(F)F.O=P(Cl)(Cl)Cl
O=C(c1c2c(cc3nc(Cl)ccc13)C1CNCC2C1)C(F)(F)F
null
null
null
Functional Group Interconversion
OtherReaction
026eb9dc25a7ccadb3fb0299071f6390008431a26aec6a612d9eb4f53467cc3c
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1cnc2cc3c(cc2c1)C1CNCC3C1
Cl-P(-Cl)(=O)-[Cl;H0;D1;+0:1].O=[c;H0;D3;+0:2]1:[c:3]:[c:4]:[c:5]:[c:6](:[c:7]):[nH;D2;+0:8]:1>>[Cl;H0;D1;+0:1]-[c;H0;D3;+0:2]1:[c:3]:[c:4]:[c:5]:[c:6](:[c:7]):[n;H0;D2;+0:8]:1
null
[]
100
CELSIUS
3
HOUR
1-(5,14-diazatetracyclo[10.3.1.02,11.04,9]hexadeca-2(11),3,7,9-tetraen-6-one-10-yl)-2,2,2-trifluoro-ethanone (156 mg, 0.49 mmol) was treated with POCl3 (5 mL) and warmed to 100° C. with stirring for 3 hours. After concentration in vacuo, the residue was diluted with CH2Cl2 (15 mL) and carefully treated with saturated N...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2cc3c(cc2n1)C1CNCC3C1
c1cnc2cc3c(cc2c1)C1CNCC3C1
c1cnc2cc3c(cc2c1)C1CNCC3C1
HCl
null
100
3
O=C(c1c2c(cc3[nH]c(=O)ccc13)C1CNCC2C1)C(F)(F)F.O=P(Cl)(Cl)Cl>>O=C(c1c2c(cc3nc(Cl)ccc13)C1CNCC2C1)C(F)(F)F
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-05d8266adde34236ba2855ba742981b5
CC(C)(C)OC(=O)c1c2c(cc3nc(Cl)ccc13)C1CNCC2C1.CO>>COc1ccc2c(C(=O)OC(C)(C)C)c3c(cc2n1)C1CNCC3C1
[Na].CO.C(C)(C)(C)OC(=O)C1=C2C=CC(=NC2=CC=2C3CNCC(C12)C3)Cl.CO>>C(C)(C)(C)OC(=O)C1=C2C=CC(=NC2=CC=2C3CNCC(C12)C3)OC
Cl[c:3]1[cH:4][cH:5][c:6]2[c:7]([C:8](=[O:9])[O:10][C:11]([CH3:12])([CH3:13])[CH3:14])[c:15]3[c:16]([cH:17][c:18]2[n:19]1)[CH:20]1[CH2:21][NH:22][CH2:23][CH:24]3[CH2:25]1.[CH3:1][OH:2]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]2[c:7]([C:8](=[O:9])[O:10][C:11]([CH3:12])([CH3:13])[CH3:14])[c:15]3[c:16]([cH:17][c:18]2[n:19]1)[C...
CC(C)(C)OC(=O)c1c2c(cc3nc(Cl)ccc13)C1CNCC2C1.CO
COc1ccc2c(C(=O)OC(C)(C)C)c3c(cc2n1)C1CNCC3C1
null
null
null
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
8c774238786d4a1a5fbc42657602149adc59fb3eba0ee102e7029b95f561c796
23dafde907f7a74dc1d4cc65967b00a9b318897fe61a3d3c4a9fddf320485f17
c1cnc2cc3c(cc2c1)C1CNCC3C1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5].[C;D1;H3:6]-[OH;D1;+0:7]>>[C;D1;H3:6]-[O;H0;D2;+0:7]-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5]
null
[]
null
null
null
null
Sodium metal (˜12 mg) was dissolved in methanol (1 mL) under nitrogen with stirring and treated with a solution of 6-chloro-5,14-diazatetracyclo[10.3.1.02,11.04,9]hexadeca-2(11),3,5,7,9-pentaen-10-carboxylic acid tert-butyl ester (118 mg, 0.33 mmol) in methanol (3 mL) and brought to reflux for 18 hours. The mixture was...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Methanol
Ether
c1cnc2cc3c(cc2c1)C1CNCC3C1
c1cnc2cc3c(cc2c1)C1CNCC3C1
c1cnc2cc3c(cc2c1)C1CNCC3C1
HCl
null
null
null
CC(C)(C)OC(=O)c1c2c(cc3nc(Cl)ccc13)C1CNCC2C1.CO>>COc1ccc2c(C(=O)OC(C)(C)C)c3c(cc2n1)C1CNCC3C1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-439e7a687fe84598b3e1c881ce019501
CC(=O)c1ccc(Br)cc1.Cc1cc(Br)ccc1C(=O)O>>O=C(CC(=O)c1ccc(Br)cc1)c1ccc(Br)cc1
CO.CC(=O)C1=CC=C(C=C1)Br.CC1=C(C(=O)O)C=CC(=C1)Br.[H-].[Na+]>>BrC1=CC=C(C=C1)C(CC(C1=CC=C(C=C1)Br)=O)=O
[CH3:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][c:9]([Br:10])[cH:11][cH:12]1.C[c:19]1[c:13]([C:2](O)=[O:1])[cH:14][cH:15][c:16]([Br:17])[cH:18]1>>[O:1]=[C:2]([CH2:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][c:9]([Br:10])[cH:11][cH:12]1)[c:13]1[cH:14][cH:15][c:16]([Br:17])[cH:18][cH:19]1
CC(=O)c1ccc(Br)cc1.Cc1cc(Br)ccc1C(=O)O
O=C(CC(=O)c1ccc(Br)cc1)c1ccc(Br)cc1
null
null
C1=CC=CC=C1
C-C Coupling
OtherReaction
8d7e298e82e4bbd5de481dd29095f1032a2d8e2f2274cb4a92b2e336e5e965b1
49910546f6df8ca015ce53553723035869f216f30f58ae8019dcd4622353d7b5
O=C(CC(=O)c1ccccc1)c1ccccc1
C-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[C;H0;D3;+0:5](-O)=[O;D1;H0:6]):[c:7].[CH3;D1;+0:8]-[C:9](=[O;D1;H0:10])-[c:11]>>[O;D1;H0:6]=[C;H0;D3;+0:5](-[CH2;D2;+0:8]-[C:9](=[O;D1;H0:10])-[c:11])-[c:4](:[c:7]):[cH;D2;+0:1]:[c:2]:[c:3]
null
[]
60
CELSIUS
null
null
In a 1-liter three neck round bottom flask, 43 g (0.2 mol) methyl 4-bromobenzoic acid and 17.6 g (0.4 mol) sodium hydride were dissolved in 200 ml dried benzene and heated to 60° C. Next, 39.8 g (0.2 mol) 4-bromoacetophenone in 100 ml dry benzene was slowly added through a dropping funnel, and 1 ml methanol was added t...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Ketone
Ketone.Ketone
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1
HO-
C1=CC=CC=C1
60
null
CC(=O)c1ccc(Br)cc1.Cc1cc(Br)ccc1C(=O)O>C1=CC=CC=C1>O=C(CC(=O)c1ccc(Br)cc1)c1ccc(Br)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-0adf17f674044210915e55a9d072a99b
NO.O=C(CC(=O)c1ccc(Br)cc1)c1ccc(Br)cc1>>Brc1ccc(-c2cc(-c3ccc(Br)cc3)on2)cc1
BrC1=CC=C(C=C1)C(CC(C1=CC=C(C=C1)Br)=O)=O.Cl.NO.[OH-].[Na+]>>BrC1=CC=C(C=C1)C1=NOC(=C1)C1=CC=C(C=C1)Br
[OH:16][NH2:17].O=[C:6]([c:5]1[cH:4][cH:3][c:2]([Br:1])[cH:19][cH:18]1)[CH2:7][C:8](=O)[c:9]1[cH:10][cH:11][c:12]([Br:13])[cH:14][cH:15]1>>[Br:1][c:2]1[cH:3][cH:4][c:5](-[c:6]2[cH:7][c:8](-[c:9]3[cH:10][cH:11][c:12]([Br:13])[cH:14][cH:15]3)[o:16][n:17]2)[cH:18][cH:19]1
NO.O=C(CC(=O)c1ccc(Br)cc1)c1ccc(Br)cc1
Brc1ccc(-c2cc(-c3ccc(Br)cc3)on2)cc1
null
null
O.O1CCOCC1
Aromatic Heterocycle Formation
OtherReaction
35a6a92be0c7e0e68e03ff68db08d05a69eb1b9c87e7a94f0e9524b2861379a6
e8142154ce82c2e242e52c937b939f3fefdc51b29f1e30581e6f69472c9bf693
c1ccc(-c2cc(-c3ccccc3)on2)cc1
O=[C;H0;D3;+0:1](-[CH2;D2;+0:2]-[C;H0;D3;+0:3](=O)-[c;H0;D3;+0:4](:[c:5]:[c:6]):[c:7]:[c:8])-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13].[NH2;D1;+0:14]-[OH;D1;+0:15]>>[c:6]:[c:5]:[c;H0;D3;+0:4](-[c;H0;D3;+0:3]1:[cH;D2;+0:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]):[n;H0;D2;+0:14]:[o;H0;D2;+0:15]:1...
null
[]
null
null
12
HOUR
In a 250 ml round bottom flask, 4 g (10.4 mmol) of [2] was dissolved in 100 ml dry dioxane and heated to reflux, then 3.0 g (43.2 mmol) hydroxylamine hydrogen chloride in 10 ml water and 5 ml (25 mmol) 5 N NaOH was then dropped into the refluxing mixture. After 12 hours, the reaction mixture was cooled down to room tem...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ketone.Primary amine
null
null
c1cnoc1
c1ccccc1.c1cnoc1.c1ccccc1
HO-
O.O1CCOCC1
null
12
NO.O=C(CC(=O)c1ccc(Br)cc1)c1ccc(Br)cc1>O.O1CCOCC1>Brc1ccc(-c2cc(-c3ccc(Br)cc3)on2)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-c817a0ea0ac64877a846f4b006c3f5c4
O=C([O-])C(=O)[O-].[Ce+3].[O-2].[O-2].[O-2]>>O=C([O-])C(=O)[O-].O=C([O-])C(=O)[O-].O=C([O-])C(=O)[O-].[Ce+3]
C(C(=O)[O-])(=O)[O-].[NH4+].[NH4+].[Cl-].[Ce+3].[Cl-].[Cl-].[O-2].[Ce+3].[O-2].[O-2].[Ce+3]>>C(C(=O)[O-])(=O)[O-].[Ce+3].C(C(=O)[O-])(=O)[O-].C(C(=O)[O-])(=O)[O-].[Ce+3]
[O:1]=[C:2]([O-:3])[C:10](=[O:11])[O-:12].[Ce+3:19].[O-2:6].[O-2:18].[O-2:5]>>[O:1]=[C:2]([O-:3])[C:4](=[O:5])[O-:6].[O:7]=[C:8]([O-:9])[C:10](=[O:11])[O-:12].[O:13]=[C:14]([O-:15])[C:16](=[O:17])[O-:18].[Ce+3:19]
O=C([O-])C(=O)[O-].[Ce+3].[O-2].[O-2].[O-2]
O=C([O-])C(=O)[O-].O=C([O-])C(=O)[O-].O=C([O-])C(=O)[O-].[Ce+3]
null
null
null
Acylation
OtherReaction
03df169542e61bc25f850d05576488c0b54839b94e3082a72ebb3e4f24252841
46615a373e6434dd65776b88d9fcc22218d37124c5265a98f610d7564f54362b
null
[O-2;H0;D0:1].[O-2;H0;D0:2].[O-2;H0;D0:3].[O;-;D1;H0:4]-[C;H0;D3;+0:5](=[O;D1;H0:6])-[C;H0;D3;+0:7](-[O;-;D1;H0:8])=[O;D1;H0:9]>>[C:10]-[C:11](-[O-;H0;D1:2])=[O;D1;H0:12].[O-;H0;D1:1]-[C:13](=[O;H0;D1;+0:3])-[C;H0;D3;+0:7](-[O;-;D1;H0:8])=[O;D1;H0:9].[O;-;D1;H0:4]-[C;H0;D3;+0:5](=[O;D1;H0:6])-[C:14](-[O;-;D1;H0:15])=[O...
null
[]
1,500
CELSIUS
null
null
A cerium oxalate powder was prepared by adding an aqueous solution of ammonium oxalate to an aqueous solution of cerium chloride under stirring, causing the precipitation of cerium oxalate, filtering, and drying. The powder was ground with a jet-mill to obtain a starting material powder with a mean particle diameter of...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
null
1,500
null
O=C([O-])C(=O)[O-].[Ce+3].[O-2].[O-2].[O-2]>>O=C([O-])C(=O)[O-].O=C([O-])C(=O)[O-].O=C([O-])C(=O)[O-].[Ce+3]
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-37e898ff656e4c9e94b943275265965e
COc1ccc(C(=O)Cl)cc1.COc1cccc(OC)c1>>COc1ccc(C(=O)c2ccc(OC)cc2OC)cc1
Cl.COC1=CC(=CC=C1)OC.C(C1=CC=C(C=C1)OC)(=O)Cl.[Cl-].[Al+3].[Cl-].[Cl-]>>COC1=C(C=CC(=C1)OC)C(=O)C1=CC=C(C=C1)OC
Cl[C:7]([c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:20][cH:19]1)=[O:8].[cH:9]1[cH:10][cH:11][c:12]([O:13][CH3:14])[cH:15][c:16]1[O:17][CH3:18]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([C:7](=[O:8])[c:9]2[cH:10][cH:11][c:12]([O:13][CH3:14])[cH:15][c:16]2[O:17][CH3:18])[cH:19][cH:20]1
COc1ccc(C(=O)Cl)cc1.COc1cccc(OC)c1
COc1ccc(C(=O)c2ccc(OC)cc2OC)cc1
null
null
C(Cl)Cl
C-C Coupling
Friedel-Crafts acylation
55541449ad4f182ef3dc0497085b282b1dcb76e0fb5ed140dc4eab4973eacb28
fe2a4a0dfbb5b71b9a065e092364c64b22b4eb1ad4d6ba2a1e8edc9d31fce3e4
O=C(c1ccccc1)c1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[#8:6]-[c:7](:[c:8]):[cH;D2;+0:9]:[c:10]:[c:11]>>[#8:6]-[c:7](:[c:8]):[c;H0;D3;+0:9](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]):[c:10]:[c:11]
null
[]
null
null
null
null
1,3-Dimethoxybenzene (13.8 g) and p-anisoyl chloride (17 g) were dissolved in a reaction flask containing 200 mL of methylene chloride and stirred at room temperature. Anhydrous aluminum chloride (15 g) was added slowly to the reaction mixture over a period of 15 minutes with stirring. After stirring an additional 15 m...
10.6084/m9.figshare.5104873.v1
null
Acyl halide
Ketone
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1
HCl
C(Cl)Cl
null
null
COc1ccc(C(=O)Cl)cc1.COc1cccc(OC)c1>C(Cl)Cl>COc1ccc(C(=O)c2ccc(OC)cc2OC)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-2b20b70246a44d1e8b70b50336b7441c
COc1ccc(C(=O)Cl)cc1.O=C(Cl)c1ccccc1F>>COc1ccc(C(=O)c2ccccc2F)cc1
C(C1=CC=C(C=C1)OC)(=O)Cl.NC1=CC=CC2=CC=CC=C12.FC1=C(C(=O)Cl)C=CC=C1.C1(=CC=CC=C1)OC>>FC1=C(C=CC=C1)C(=O)C1=CC=C(C=C1)OC
O=C(Cl)[c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:17][cH:16]1.Cl[C:7](=[O:8])[c:9]1[cH:10][cH:11][cH:12][cH:13][c:14]1[F:15]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([C:7](=[O:8])[c:9]2[cH:10][cH:11][cH:12][cH:13][c:14]2[F:15])[cH:16][cH:17]1
COc1ccc(C(=O)Cl)cc1.O=C(Cl)c1ccccc1F
COc1ccc(C(=O)c2ccccc2F)cc1
null
null
null
C-C Coupling
OtherReaction
2141d805cb200c555dd0a65a475dafdab76558b89bb294884d98559bfa317f3e
75a41004d03d2a6fb764d4720e5d90b58a710658470b24716bc9c18b018af260
O=C(c1ccccc1)c1ccccc1
Cl-C(=O)-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].Cl-[C;H0;D3;+0:6](=[O;D1;H0:7])-[c:8](:[c:9]):[c:10]>>[O;D1;H0:7]=[C;H0;D3;+0:6](-[c:8](:[c:9]):[c:10])-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
null
[]
null
null
null
null
The procedure of Example 10 was followed except as follows. In Part A, 1-amino napthalene (47 g) was used in place of 4-methoxy aniline. In Step 1 of Part B, 2-fluorobenzoyl chloride (15.8 g) and anisole (10.8 g) were used in place of 1,3-dimethoxybenezene and p-anisoyl chloride respectively to produce (2-fluoro-phenyl...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Acyl halide
Ketone
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1
Other
null
null
null
COc1ccc(C(=O)Cl)cc1.O=C(Cl)c1ccccc1F>>COc1ccc(C(=O)c2ccccc2F)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-dfe4ced729254e01be55cc9bea0175d5
O=C(O)c1ccc(O)cc1.OCCCCCCCl>>O=C(O)c1ccc(OCCCCCCO)cc1
OC1=CC=C(C(=O)O)C=C1.ClCCCCCCO>>OCCCCCCOC1=CC=C(C(=O)O)C=C1
[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][c:7]([OH:8])[cH:16][cH:17]1.Cl[CH2:9][CH2:10][CH2:11][CH2:12][CH2:13][CH2:14][OH:15]>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][c:7]([O:8][CH2:9][CH2:10][CH2:11][CH2:12][CH2:13][CH2:14][OH:15])[cH:16][cH:17]1
O=C(O)c1ccc(O)cc1.OCCCCCCCl
O=C(O)c1ccc(OCCCCCCO)cc1
null
null
[OH-].[K+]
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
7e1040116e3a4cf0e8ec5cc7865388d9cd0efabce6d320a1c25a36e411018d8b
d5f4610d46ccc0478471c5bc0fb862644eaf764bbc5d93badb39d54f6ec8e0a5
c1ccccc1
Cl-[CH2;D2;+0:1]-[C:2]-[C:3].[OH;D1;+0:4]-[c:5](:[c:6]):[c:7]>>[C:3]-[C:2]-[CH2;D2;+0:1]-[O;H0;D2;+0:4]-[c:5](:[c:6]):[c:7]
80
[{"value": 80.0, "product": "OCCCCCCOC1=CC=C(C(=O)O)C=C1", "details": "PERCENTYIELD", "is_desired": false}]
60
CELSIUS
null
null
Monomers in which the bulky organic group was a t-butyl group and the alkyl groups were hexyl groups were made as follows. 4-hydroxybenzoic acid was dissolved in 30% ethanolic KOH. About 1% of KI was added as a catalyst. The mixture was heated to about 60° C. and a stoichiometric amount of 6-chloro-1-hexanol was slowly...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic alcohol
Ether
null
null
c1ccccc1
HCl
[OH-].[K+]
60
null
O=C(O)c1ccc(O)cc1.OCCCCCCCl>[OH-].[K+]>O=C(O)c1ccc(OCCCCCCO)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-6961669486c8494bb2c3a3bdd60048e7
NC(=O)c1ccncc1>>NC(=O)c1ccncc1
C1=C(N=C(S1)NC(=N)N)CSCCC(=N)NS(=O)(=O)N.C1=C(N=C(S1)NC(=N)N)CSCCC(=N)NS(=O)(=O)N.C(C1=CC=NC=C1)(=O)N.C(C(O)C)(=O)O>>C(C1=CC=NC=C1)(=O)N.C(C(O)C)(=O)O
[NH2:7][C:8](=[O:9])[c:10]1[cH:11][cH:12][n:13][cH:14][cH:15]1>>[NH2:7][C:8](=[O:9])[c:10]1[cH:11][cH:12][n:13][cH:14][cH:15]1
NC(=O)c1ccncc1
NC(=O)c1ccncc1
null
null
O
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
c1ccncc1
null
null
[]
null
null
null
null
To 1 g of famotidine and 5 g of isonicotinic acid amide were added about 80 ml of water for injection and 2.20 ml of a 100 mg/ml aqueous lactic acid solution, followed by stirring to dissolve them. After complete dissolution of famotidine, water for injection was added to make the total volume 100 ml, whereby an inject...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
c1ccncc1
null
O
null
null
NC(=O)c1ccncc1>O>NC(=O)c1ccncc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-4f7b41588ad642d29308ad28a09d5a18
Cc1ccc2sc3cc(C(=O)O)ccc3c(=O)c2c1.O=S(Cl)Cl>>Cc1ccc2sc3cc(C(=O)Cl)ccc3c(=O)c2c1
CC1=CC=C2SC=3C=C(C=CC3C(C2=C1)=O)C(=O)O.S(=O)(Cl)Cl.CN(C=O)C>>CC1=CC=C2SC=3C=C(C=CC3C(C2=C1)=O)C(=O)Cl
O[C:10]([c:9]1[cH:8][c:7]2[s:6][c:5]3[cH:4][cH:3][c:2]([CH3:1])[cH:19][c:18]3[c:16](=[O:17])[c:15]2[cH:14][cH:13]1)=[O:11].O=S(Cl)[Cl:12]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]2[s:6][c:7]3[cH:8][c:9]([C:10](=[O:11])[Cl:12])[cH:13][cH:14][c:15]3[c:16](=[O:17])[c:18]2[cH:19]1
Cc1ccc2sc3cc(C(=O)O)ccc3c(=O)c2c1.O=S(Cl)Cl
Cc1ccc2sc3cc(C(=O)Cl)ccc3c(=O)c2c1
null
null
C1(=CC=CC=C1)C
Functional Group Interconversion
Alcohol to chloride_SOCl2
c301c14a9dcd0670d52e8b77396cbe7fd8edeedd757bc43f4162ade1fc52fc93
787f545db5dc0b29dde55b5fbed7db8625b8055f49327f97ed4d83cc47c3af1d
O=c1c2ccccc2sc2ccccc12
Cl-S(=O)-[Cl;H0;D1;+0:1].O-[C;H0;D3;+0:2](=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[c:7]:[#16;a:8]>>[#16;a:8]:[c:7]:[c:6]:[c:4](-[C;H0;D3;+0:2](-[Cl;H0;D1;+0:1])=[O;D1;H0:3]):[c:5]
85
[{"value": 85.0, "product": "CC1=CC=C2SC=3C=C(C=CC3C(C2=C1)=O)C(=O)Cl", "details": "PERCENTYIELD", "is_desired": false}]
null
null
16
HOUR
The 7-methyl-9-oxothioxanthene-3-carboxylic acid (MTA), 50.0 g (0.185 mol), was dissolved in 350 ml of toluene and 415 ml (5.69 mol) of thionyl chloride using an overhead stirrer in a 2 liter 3-neck round bottom flask. N,N-Dimethylformamide (DMF), 2 ml, was added and the reaction was brought to reflux for 2 hours. Afte...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Acyl halide
null
null
c1ccc2sc3ccccc3cc2c1
HCl
C1(=CC=CC=C1)C
null
16
Cc1ccc2sc3cc(C(=O)O)ccc3c(=O)c2c1.O=S(Cl)Cl>C1(=CC=CC=C1)C>Cc1ccc2sc3cc(C(=O)Cl)ccc3c(=O)c2c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-21dd6ba93a02489eb74c79b936dfe3ac
CC(=O)OC(C)=O.O=C(O)/C=C\C(=O)NCCCCCC(=O)O.c1ccc2c(c1)Nc1ccccc1S2>>O=C(CCCCCN1C(=O)C=CC1=O)ON1C(=O)CCC1=O
O=C(\C=C/C(=O)O)NCCCCCC(=O)O.C(C)(=O)OC(C)=O.C1=CC=CC=2SC3=CC=CC=C3NC12.Cl.O>>C1CC(=O)N(C1=O)OC(=O)CCCCCN2C(=O)C=CC2=O
CC(=O)OC(C)=[O:18].[O:1]=[C:2]([CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][NH:8][C:13](/[CH:12]=[CH:11]\[C:9](=[O:10])[OH:22])=[O:14])[OH:15].c1cc[c:21]2c(c1)Sc1cc[cH:20][cH:19][c:17]1[NH:16]2>>[O:1]=[C:2]([CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][N:8]1[C:9](=[O:10])[CH:11]=[CH:12][C:13]1=[O:14])[O:15][N:16]1[C:17](=[O:18])[CH2:19][...
CC(=O)OC(C)=O.O=C(O)/C=C\C(=O)NCCCCCC(=O)O.c1ccc2c(c1)Nc1ccccc1S2
O=C(CCCCCN1C(=O)C=CC1=O)ON1C(=O)CCC1=O
null
null
C1CCOC1.C(C)N(CC)CC
C-C Coupling
OtherReaction
6db43b436ba612c61d3a5f5367e148113f0fee4b92812126b59adc2e26919ec0
669dea8e1aa93881007fcd6c4da5254692628cb2aef0cdc3dbd59cf58249f8d6
O=C(CCCCCN1C(=O)C=CC1=O)ON1C(=O)CCC1=O
C-C(=O)-O-C(-C)=[O;H0;D1;+0:1].S1-c2:c:c:[cH;D2;+0:2]:[cH;D2;+0:3]:[c;H0;D3;+0:4]:2-[NH;D2;+0:5]-[c;H0;D3;+0:6]2:c:c:c:c:c:2-1.[C:7]-[C:8](=[O;D1;H0:9])-[OH;D1;+0:10].[C:11]-[C:12]-[NH;D2;+0:13]-[C:14](=[O;D1;H0:15])/[C:16]=[C:17]\[C;H0;D3;+0:18](=[O;D1;H0:19])-[OH;D1;+0:20]>>[C:7]-[C:8](=[O;D1;H0:9])-[O;H0;D2;+0:10]-[...
null
[]
null
null
null
null
(Z)-4-Oxo-5-aza-2-undecendioic acid, 150.0 g (0.654 moles), acetic anhydride, 68 ml (73.5 g, 0.721 moles), and phenothiazine, 500 mg, were added to a 2 liter three-neck round bottom flask equipped with an overhead stirrer. Triethylamine, 91 ml (0.653 moles), and 600 ml of THF were added and the mixture was heated to re...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Carboxylic acid.Carboxylic acid.Secondary amide.Secondary amine.Monosulfide
Substituted dicarboximide.Tertiary amide.Tertiary amide
c1ccc2c(c1)Nc1ccccc1S2
C1=CC[NH]C1.C1CC[NH]C1
C1=CC[NH]C1.C1CC[NH]C1
Other
C1CCOC1.C(C)N(CC)CC
null
null
CC(=O)OC(C)=O.O=C(O)/C=C\C(=O)NCCCCCC(=O)O.c1ccc2c(c1)Nc1ccccc1S2>C1CCOC1.C(C)N(CC)CC>O=C(CCCCCN1C(=O)C=CC1=O)ON1C(=O)CCC1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-8515cfed68d2474e998cef70299e4581
COc1ccc(C(C)=O)cc1.O=C/C=C/c1ccccc1>>COc1ccc(C(=O)C=CC=Cc2ccccc2)cc1
C(\C=C\C1=CC=CC=C1)=O.CC(=O)C1=CC=C(C=C1)OC.[OH-].[Na+]>>COC1=CC=C(C=C1)C(C=CC=CC1=CC=CC=C1)=O
[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([C:7](=[O:8])[CH3:9])[cH:19][cH:20]1.O=[CH:10]/[CH:11]=[CH:12]/[c:13]1[cH:14][cH:15][cH:16][cH:17][cH:18]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([C:7](=[O:8])[CH:9]=[CH:10][CH:11]=[CH:12][c:13]2[cH:14][cH:15][cH:16][cH:17][cH:18]2)[cH:19][cH:20]1
COc1ccc(C(C)=O)cc1.O=C/C=C/c1ccccc1
COc1ccc(C(=O)C=CC=Cc2ccccc2)cc1
null
null
C(C)O
C-C Coupling
Aldehyde and ketone to alpha,beta-unsaturated carbonyl
f500c100f5cd3378729ee1542c3d95141e4f1833211cc2ce0c35099b4e896130
101c8d17ab7e80420efd3d968b7962dd5450cc718389428be42f0baaa6391f61
O=C(C=CC=Cc1ccccc1)c1ccccc1
O=[CH;D2;+0:1]/[C:2]=[C:3]/[c:4](:[c:5]):[c:6].[CH3;D1;+0:7]-[C:8](=[O;D1;H0:9])-[c:10]>>[O;D1;H0:9]=[C:8](-[c:10])-[CH;D2;+0:7]=[CH;D2;+0:1]-[C:2]=[C:3]-[c:4](:[c:5]):[c:6]
72
[{"value": 72.0, "product": "COC1=CC=C(C=C1)C(C=CC=CC1=CC=CC=C1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
12
HOUR
2 ml of trans-cinnamaldehyde and 2.5 g of 4-methoxy acetophenone were dissolved in 50 ml of ethanol at room temperature. 10 ml of sodium hydroxide solution was then added and stirred for 12 h to form yellow solid precipitation. Filtering the precipitation to obtain the compound 1, with yield of 72% and purity of 96.3%....
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Ketone
Ketone.Conjugated diene
null
null
c1ccccc1.c1ccccc1
HO-
C(C)O
null
12
COc1ccc(C(C)=O)cc1.O=C/C=C/c1ccccc1>C(C)O>COc1ccc(C(=O)C=CC=Cc2ccccc2)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-bbc38cb4d21e4dbba0e6138c6543b664
O=C(O)c1ccccc1-c1ccccc1C(=O)O>>O=C(O)c1cccc2c1-c1ccccc1C2=O
C=1(C(C(=O)O)=CC=CC1)C=1C(C(=O)O)=CC=CC1>>C1=CC=C2C(=C1)C3=C(C2=O)C=CC=C3C(=O)O
O=[C:16]([c:15]1[c:10](-[c:9]2[c:4]([C:2](=[O:1])[OH:3])[cH:5][cH:6][cH:7][cH:8]2)[cH:11][cH:12][cH:13][cH:14]1)[OH:17]>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][cH:7][c:8]2[c:9]1-[c:10]1[cH:11][cH:12][cH:13][cH:14][c:15]1[C:16]2=[O:17]
O=C(O)c1ccccc1-c1ccccc1C(=O)O
O=C(O)c1cccc2c1-c1ccccc1C2=O
null
null
S(O)(O)(=O)=O
Functional Group Interconversion
OtherReaction
7ef164e95534b750b8f447337d5960d1ddb5d629daec09f6c5afef2d8b94fe7a
6a71bb5a71b59feeb4f6a39b1b66fa450a058b64b0a3909e1a51c22473a141c5
O=C1c2ccccc2-c2ccccc21
O=[C;H0;D3;+0:1](-[OH;D1;+0:2])-[c:3](:[c:4]):[c:5]-[c:6](:[c:7]-[C:8](=[O;D1;H0:9])-[O;D1;H1:10]):[cH;D2;+0:11]:[c:12]:[c:13]>>[O;D1;H0:9]=[C:8](-[O;D1;H1:10])-[c:7]:[c:6]1:[c;H0;D3;+0:11](:[c:12]:[c:13])-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3](:[c:4]):[c:5]-1
null
[]
70
CELSIUS
null
null
The following steps are suitable for synthesizing some charge transport materials of this invention involving a linking reaction as described in the following. In the first step, diphenic acid or its derivative is dissolved in large access of concentrated sulfuric acid and the solution is heated at approximately 70° C....
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Ketone
c1ccccc1
c1ccc2c(c1)Cc1ccccc12
c1ccc2c(c1)Cc1ccccc12
HO-
S(O)(O)(=O)=O
70
null
O=C(O)c1ccccc1-c1ccccc1C(=O)O>S(O)(O)(=O)=O>O=C(O)c1cccc2c1-c1ccccc1C2=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-b44b058630ea4732a4877a0e475a05d2
O=C(O)c1cccc2c1-c1ccccc1C2=O.O=S(Cl)Cl>>O=C(Cl)c1cccc2c1-c1ccccc1C2=O
C1=CC=C2C(=C1)C3=C(C2=O)C=CC=C3C(=O)O.S(=O)(Cl)Cl>>C1=CC=C(C=2C3=CC=CC=C3C(C12)=O)C(=O)Cl
O[C:2](=[O:1])[c:4]1[cH:5][cH:6][cH:7][c:8]2[c:9]1-[c:10]1[cH:11][cH:12][cH:13][cH:14][c:15]1[C:16]2=[O:17].O=S(Cl)[Cl:3]>>[O:1]=[C:2]([Cl:3])[c:4]1[cH:5][cH:6][cH:7][c:8]2[c:9]1-[c:10]1[cH:11][cH:12][cH:13][cH:14][c:15]1[C:16]2=[O:17]
O=C(O)c1cccc2c1-c1ccccc1C2=O.O=S(Cl)Cl
O=C(Cl)c1cccc2c1-c1ccccc1C2=O
null
null
null
Functional Group Interconversion
Alcohol to chloride_SOCl2
c301c14a9dcd0670d52e8b77396cbe7fd8edeedd757bc43f4162ade1fc52fc93
787f545db5dc0b29dde55b5fbed7db8625b8055f49327f97ed4d83cc47c3af1d
O=C1c2ccccc2-c2ccccc21
Cl-S(=O)-[Cl;H0;D1;+0:1].O-[C;H0;D3;+0:2](=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]>>[Cl;H0;D1;+0:1]-[C;H0;D3;+0:2](=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]
null
[]
null
null
null
null
The following steps are suitable for synthesizing some charge transport materials of this invention involving a linking reaction as described in the following. In the first step, diphenic acid or its derivative is dissolved in large access of concentrated sulfuric acid and the solution is heated at approximately 70° C....
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Acyl halide
null
null
c1ccc2c(c1)Cc1ccccc12
HCl
null
null
null
O=C(O)c1cccc2c1-c1ccccc1C2=O.O=S(Cl)Cl>>O=C(Cl)c1cccc2c1-c1ccccc1C2=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-5934e900187f46f2962c30933ab22f3e
NC(CO)(CO)CO.O=C[C@H](O)[C@@H](O)[C@H](O)[C@H](O)CO.O=P([O-])(O)O>>N[C@H]1C(O)O[C@H](COP(=O)(O)O)[C@@H](O)[C@@H]1O
OP(=O)(O)[O-].[K+].[Na+].[Cl-].C(CC(O)(C(=O)O)CC(=O)O)(=O)O.O=C[C@H](O)[C@@H](O)[C@H](O)[C@H](O)CO.C(C(CO)(CO)N)O.[NH4+].[OH-]>>P(=O)(O)(O)OC[C@@H]1[C@H]([C@@H]([C@H](C(O)O1)N)O)O
OC[C:2](CO)([NH2:1])[CH2:3][OH:4].OC[C@@H](O)[C@H:15]([C@@H:13]([C@@H:6]([OH:5])[CH:7]=[O:8])[OH:14])[OH:16].[O-][P:9](=[O:10])([OH:11])[OH:12]>>[NH2:1][C@H:2]1[CH:3]([OH:4])[O:5][C@H:6]([CH2:7][O:8][P:9](=[O:10])([OH:11])[OH:12])[C@@H:13]([OH:14])[C@@H:15]1[OH:16]
NC(CO)(CO)CO.O=C[C@H](O)[C@@H](O)[C@H](O)[C@H](O)CO.O=P([O-])(O)O
N[C@H]1C(O)O[C@H](COP(=O)(O)O)[C@@H](O)[C@@H]1O
null
[O-]S(=O)(=O)[O-].[Mn+2].O
null
Heteroatom Alkylation and Arylation
OtherReaction
1b9daa8571298221fc3f0f80f38b01eb9c8fd4973f6f786c32e86dbcb530321d
f450bbdca41fe80f7e780f687ed680a7c86943e5b833f2419f80307e98e9aa07
C1CCOCC1
O-C-[C;H0;D4;+0:1](-[N;D1;H2:2])(-C-O)-[CH2;D2;+0:3]-[O;D1;H1:4].O-C-[C@@H](-O)-[C@@H;D3;+0:5](-[O;D1;H1:6])-[C:7](-[O;D1;H1:8])-[C:9](-[OH;D1;+0:10])-[CH;D2;+0:11]=[O;H0;D1;+0:12].[O-]-[P;H0;D4;+0:13](=[O;D1;H0:14])(-[O;D1;H1:15])-[O;D1;H1:16]>>[N;D1;H2:2]-[C@@H;D3;+0:1]1-[C@@H;D3;+0:5](-[O;D1;H1:6])-[C:7](-[O;D1;H1:8...
null
[]
null
null
24
HOUR
coli cells from frozen vials were inoculated into a flask culture containing 12 L fermentation seed medium. The medium contained the following chemicals (g/L): corn steep liquor, 10; KH2PO4, 2.5; MgSO4.7H2O, 2.0; (NH4)2SO4, 0.5; citric acid, 0.192; FeSO4.7H2O, 0.03; MnSO4.H2O, 0.021; antifoam 6000K, 0.5; dextrose, 84. ...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary alcohol.Primary alcohol.Primary alcohol.Primary alcohol.Secondary alcohol.Secondary alcohol.Secondary alcohol
Ether.Secondary alcohol.Secondary alcohol.Phosphate ester
null
C1CCOCC1
C1CCOCC1
HO-
[O-]S(=O)(=O)[O-].[Mn+2].O
null
24
NC(CO)(CO)CO.O=C[C@H](O)[C@@H](O)[C@H](O)[C@H](O)CO.O=P([O-])(O)O>[O-]S(=O)(=O)[O-].[Mn+2].O>N[C@H]1C(O)O[C@H](COP(=O)(O)O)[C@@H](O)[C@@H]1O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-fbe48744c0294939ba6d1cf3cf9c9148
CC1(C)S[C@@H]2[C@H](NC(=O)[C@H](N)c3ccccc3)C(=O)N2[C@H]1C(=O)O.CN(C)[C@@H]1C(O)=C(C(N)=O)C(=O)[C@@]2(O)C(O)=C3C(=O)c4c(O)cccc4[C@@](C)(O)[C@H]3C[C@@H]12>>C[C@H](O)[C@H](O)[C@@H](O)[C@@H](O)C=O
C[C@]1(C=2C=CC=C(C2C(=O)C3=C([C@]4([C@@H](C[C@@H]31)[C@@H](C(=C(C4=O)C(=O)N)O)N(C)C)O)O)O)O.CC1([C@@H](N2[C@H](S1)[C@@H](C2=O)NC(=O)[C@@H](C=3C=CC=CC3)N)C(=O)O)C>>O=C[C@H](O)[C@H](O)[C@@H](O)[C@@H](O)C
CC1(C)S[C@@H]2[C@H](NC(=O)[C@H](N)c3ccccc3)C(=O)N2[C@H:8]1[C:10](=O)[OH:11].CN(C)[C@@H]1C([OH:5])=C(C(N)=O)C(=O)[C@@:6]2([OH:7])C([OH:9])=C3C(=O)c4c(O)cccc4[C@@:2]([CH3:1])([OH:3])[C@H:4]3C[C@@H]12>>[CH3:1][C@H:2]([OH:3])[C@H:4]([OH:5])[C@@H:6]([OH:7])[C@@H:8]([OH:9])[CH:10]=[O:11]
CC1(C)S[C@@H]2[C@H](NC(=O)[C@H](N)c3ccccc3)C(=O)N2[C@H]1C(=O)O.CN(C)[C@@H]1C(O)=C(C(N)=O)C(=O)[C@@]2(O)C(O)=C3C(=O)c4c(O)cccc4[C@@](C)(O)[C@H]3C[C@@H]12
C[C@H](O)[C@H](O)[C@@H](O)[C@@H](O)C=O
null
null
null
Acylation
OtherReaction
684f06e05d012b9e101b6ece1a91fbd4be217656196f53791cc06681757be199
79340e30ff356cc2f5a500bf7fcf29daef145103f8b1fd59f21154fcea797f4a
null
null
null
[]
null
null
null
null
The plasmid pBRsacH3 (Example 1) was used for cloning the rMET1 antibody (Example 9). In this case, the kappa and heavy chains were engineered with human ceruloplasmin and human neutrophil defensin signal sequences, respectively (Example 9). This plasmid was electroporated into E. coli strain DH10B rha+ to generate clo...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Ketone.Ketone.Primary amide.Secondary amide.Tertiary amide.Tertiary alcohol.Tertiary alcohol.Aromatic alcohol.Enol.Enol.Primary amine.Tertiary amine.Monosulfide
Aldehyde.Secondary alcohol.Secondary alcohol.Secondary alcohol.Secondary alcohol
c1ccccc1.C1CN2CC[C@H]2S1.C1=CC[C@H]2C=C3Cc4ccccc4C[C@H]3C[C@H]2C1
null
null
Other
null
null
null
CC1(C)S[C@@H]2[C@H](NC(=O)[C@H](N)c3ccccc3)C(=O)N2[C@H]1C(=O)O.CN(C)[C@@H]1C(O)=C(C(N)=O)C(=O)[C@@]2(O)C(O)=C3C(=O)c4c(O)cccc4[C@@](C)(O)[C@H]3C[C@@H]12>>C[C@H](O)[C@H](O)[C@@H](O)[C@@H](O)C=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-afeca0c943ca41f0aa079e3950bd9291
CC(=O)OC(C)(C)C.O=C1C[C@H](O)CO1>>CC(C)(C)OC(=O)CC(=O)C[C@H](O)CO
C(C)(C)[N-]C(C)C.[Li+].C(C)(C)[N-]C(C)C.[Li+].C(CCC)[Li].C(C)(C)NC(C)C.Cl.O[C@H]1CC(=O)OC1.C(C)(=O)OC(C)(C)C>>C(C)(C)(C)OC(CC(C[C@@H](CO)O)=O)=O
[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH3:8].[C:9]1(=[O:10])[CH2:11][C@H:12]([OH:13])[CH2:14][O:15]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][C:9](=[O:10])[CH2:11][C@H:12]([OH:13])[CH2:14][OH:15]
CC(=O)OC(C)(C)C.O=C1C[C@H](O)CO1
CC(C)(C)OC(=O)CC(=O)C[C@H](O)CO
null
null
C(C)(=O)OCC.O1CCCC1.CCCCCC
C-C Coupling
OtherReaction
6101cad8e2935c8b5c0ac7b0e1858cf3a3d323219bb17c58420a61905745e852
1002d3291f2ad18779eb4fab129659f5bfd76d885e10bba8befbd85b6c532bbb
null
[C;D1;H3:1]-[C:2](-[C;D1;H3:3])(-[C;D1;H3:4])-[#8:5]-[C:6](-[CH3;D1;+0:7])=[O;D1;H0:8].[O;D1;H0:9]=[C;H0;D3;+0:10]1-[C:11]-[C:12]-[C:13]-[O;H0;D2;+0:14]-1>>[C;D1;H3:1]-[C:2](-[C;D1;H3:3])(-[C;D1;H3:4])-[#8:5]-[C:6](=[O;D1;H0:8])-[CH2;D2;+0:7]-[C;H0;D3;+0:10](=[O;D1;H0:9])-[C:11]-[C:12]-[C:13]-[OH;D1;+0:14]
6
[{"value": 6.0, "product": "C(C)(C)(C)OC(CC(C[C@@H](CO)O)=O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 5.7, "product": "C(C)(C)(C)OC(CC(C[C@@H](CO)O)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
5
CELSIUS
null
null
To 30 mL (45 mmol) of a solution of n-butyllithium in hexane (1.5 mol/L) was added a solution of diisopropylamine (5.01 g, 49.5 mmol)-tetrahydrofuran (5 mL) dropwise under stirring at 5° C., and the mixture was stirred under argon for 1 hour to prepare a lithium diisopropylamide solution. In a separate vessel, 1.02 g (...
10.6084/m9.figshare.5104873.v1
null
Ester.Ester
Ketone.Ester.Primary alcohol
C1CCOC1
null
null
null
C(C)(=O)OCC.O1CCCC1.CCCCCC
5
null
CC(=O)OC(C)(C)C.O=C1C[C@H](O)CO1>C(C)(=O)OCC.O1CCCC1.CCCCCC>CC(C)(C)OC(=O)CC(=O)C[C@H](O)CO
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-1fa056755395410a8769840af876295d
CC(C)(C)OC(=O)CBr.O=C1C[C@H](O)CO1>>CC(C)(C)OC(=O)CC(=O)C[C@H](O)CO
BrCC(=O)OC(C)(C)C.C[Si](C)(C)Cl.BrCC(=O)OC(C)(C)C.O[C@H]1CC(=O)OC1.[OH-].[Na+]>>C(C)(C)(C)OC(CC(C[C@@H](CO)O)=O)=O
Br[CH2:8][C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7].[C:9]1(=[O:10])[CH2:11][C@H:12]([OH:13])[CH2:14][O:15]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][C:9](=[O:10])[CH2:11][C@H:12]([OH:13])[CH2:14][OH:15]
CC(C)(C)OC(=O)CBr.O=C1C[C@H](O)CO1
CC(C)(C)OC(=O)CC(=O)C[C@H](O)CO
null
[Zn]
O.O1CCCC1
C-C Coupling
OtherReaction
c6f8192bbe03a14b72dd6a446dcadca28ed9a702b97f7f2c9f67505ce87241e7
927029737ca4800f17176897b097086b9e9024d361c17b2cd676dad17a2af962
null
Br-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#8:4]-[C:5](-[C;D1;H3:6])(-[C;D1;H3:7])-[C;D1;H3:8].[O;D1;H0:9]=[C;H0;D3;+0:10]1-[C:11]-[C:12]-[C:13]-[O;H0;D2;+0:14]-1>>[C;D1;H3:6]-[C:5](-[C;D1;H3:7])(-[C;D1;H3:8])-[#8:4]-[C:2](=[O;D1;H0:3])-[CH2;D2;+0:1]-[C;H0;D3;+0:10](=[O;D1;H0:9])-[C:11]-[C:12]-[C:13]-[OH;D1;+0:14]
116.1
[{"value": 29.0, "product": "C(C)(C)(C)OC(CC(C[C@@H](CO)O)=O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 116.1, "product": "C(C)(C)(C)OC(CC(C[C@@H](CO)O)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
65
CELSIUS
30
MINUTE
To a suspension of 9.82 g (150 mmol) of zinc dust in 40 mL of tetrahydrofuran was added 1.9 mL (15 mmol) of trimethylsilyl chloride at room temperature, and the mixture was stirred for 30 minutes. To this mixture were added 2.4 mL (10.5 mmol) of tert-butyl α-bromoacetate and 4.27 g (42 mmol) of (S)-β-hydroxy-γ-butyrola...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester.Ester
Ketone.Ester.Primary alcohol
C1CCOC1
null
null
Br-
[Zn].O.O1CCCC1
65
0.5
CC(C)(C)OC(=O)CBr.O=C1C[C@H](O)CO1>[Zn].O.O1CCCC1>CC(C)(C)OC(=O)CC(=O)C[C@H](O)CO
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-29050331286246aa9b5102f1f43d720f
CC(C)(C)OC(=O)CC(=O)C[C@H](O)CO.O=C(Cl)c1ccccc1>>CC(C)(C)OC(=O)CC(=O)C[C@H](O)COC(=O)c1ccccc1
[OH-].[Na+].C(C)(C)(C)OC(CC(C[C@@H](CO)O)=O)=O.N1=CC=CC=C1.C(C1=CC=CC=C1)(=O)Cl>>C(C)(C)(C)OC(CC(C[C@@H](COC(C1=CC=CC=C1)=O)O)=O)=O
[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][C:9](=[O:10])[CH2:11][C@H:12]([OH:13])[CH2:14][OH:15].Cl[C:16](=[O:17])[c:18]1[cH:19][cH:20][cH:21][cH:22][cH:23]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][C:9](=[O:10])[CH2:11][C@H:12]([OH:13])[CH2:14][O:15][C:16](=[O:17])[c:18]1[cH:19][cH:20][cH:...
CC(C)(C)OC(=O)CC(=O)C[C@H](O)CO.O=C(Cl)c1ccccc1
CC(C)(C)OC(=O)CC(=O)C[C@H](O)COC(=O)c1ccccc1
null
null
O.C(Cl)Cl
Acylation
Schotten-Baumann to ester
6cefe709828c5bd4655f254e75d5dff9e8876e192e7dd47256c1bc0067bc5291
d8a7643b81ed07a6f633aa99465180dfa0565e61ae25aef36338ebb9837c9cef
c1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C:6]-[C:7]-[OH;D1;+0:8]>>[C:6]-[C:7]-[O;H0;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
78
[{"value": 78.0, "product": "C(C)(C)(C)OC(CC(C[C@@H](COC(C1=CC=CC=C1)=O)O)=O)=O", "details": "PERCENTYIELD", "is_desired": false}]
0
CELSIUS
2
HOUR
To a solution of 16.8 g (77 mmol) of the (5S)-5,6-dihydroxy-3-oxohexanoic tert-butyl ester produced in Example 1 in 120 mL of methylene chloride were added 11.2 mL of pyridine and 10.2 mL of benzoyl chloride at 0° C., and the mixture was stirred at 0° C. for 2 hours. After completion of the reaction, the reaction mixtu...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary alcohol
Ester
null
null
c1ccccc1
HCl
O.C(Cl)Cl
0
2
CC(C)(C)OC(=O)CC(=O)C[C@H](O)CO.O=C(Cl)c1ccccc1>O.C(Cl)Cl>CC(C)(C)OC(=O)CC(=O)C[C@H](O)COC(=O)c1ccccc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-26bcb764111141deba45aba2d82d8f7e
CC(C)(C)OC(=O)CC(=O)C[C@H](O)COC(=O)c1ccccc1>>CC(C)(C)OC(=O)C[C@H](O)C[C@H](O)COC(=O)c1ccccc1
C(C)(C)(C)OC(CC(C[C@@H](COC(C1=CC=CC=C1)=O)O)=O)=O.O=C[C@H](O)[C@@H](O)[C@H](O)[C@H](O)CO.C(C)(=O)OCC>>C(C)(C)(C)OC(C[C@@H](C[C@@H](COC(C1=CC=CC=C1)=O)O)O)=O
[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][C:9](=[O:10])[CH2:11][C@H:12]([OH:13])[CH2:14][O:15][C:16](=[O:17])[c:18]1[cH:19][cH:20][cH:21][cH:22][cH:23]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][C@H:9]([OH:10])[CH2:11][C@H:12]([OH:13])[CH2:14][O:15][C:16](=[O:17])[c:18]1[cH:19][cH:20][cH:21...
CC(C)(C)OC(=O)CC(=O)C[C@H](O)COC(=O)c1ccccc1
CC(C)(C)OC(=O)C[C@H](O)C[C@H](O)COC(=O)c1ccccc1
null
null
P(=O)([O-])([O-])[O-]
Reduction
Reduction of ketone to secondary alcohol
02790ac194d8bf7ccb13d6247c59412024d87f77d2c906ef7804f021f57d5070
1bd3cd74b454139c0a0068ac0135836499926b274bff569df163210c6c944a89
c1ccccc1
[C:1]-[C:2]-[C;H0;D3;+0:3](=[O;H0;D1;+0:4])-[C:5]-[C:6](=[O;D1;H0:7])-[#8:8]-[C:9](-[C;D1;H3:10])(-[C;D1;H3:11])-[C;D1;H3:12]>>[C:1]-[C:2]-[C@@H;D3;+0:3](-[OH;D1;+0:4])-[C:5]-[C:6](=[O;D1;H0:7])-[#8:8]-[C:9](-[C;D1;H3:10])(-[C;D1;H3:11])-[C;D1;H3:12]
null
[]
27
CELSIUS
2.5
DAY
A large test tube was charged with 5 ml of Medium A described hereinbefore and, after sterilization, inoculated with one of the microorganisms indicated in Table 1 and Table 2. Aerobic shake culture was carried out at 27° C. for 2 to 3 days. From a 1.5 ml portion of the resulting culture, the cells were harvested by ce...
10.6084/m9.figshare.5104873.v1
null
Ketone
Secondary alcohol
null
null
c1ccccc1
null
P(=O)([O-])([O-])[O-]
27
60
CC(C)(C)OC(=O)CC(=O)C[C@H](O)COC(=O)c1ccccc1>P(=O)([O-])([O-])[O-]>CC(C)(C)OC(=O)C[C@H](O)C[C@H](O)COC(=O)c1ccccc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-bf0fdec98e874af7be6a18c9a6110a97
CC(C)(C)OC(=O)CC(=O)C[C@H](O)COC(=O)c1ccccc1>>CC(C)(C)OC(=O)C[C@H](O)C[C@H](O)COC(=O)c1ccccc1
C(C)(C)(C)OC(CC(C[C@@H](COC(C1=CC=CC=C1)=O)O)=O)=O.O=C[C@H](O)[C@@H](O)[C@H](O)[C@H](O)CO>>C(C)(C)(C)OC(C[C@@H](C[C@@H](COC(C1=CC=CC=C1)=O)O)O)=O
[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][C:9](=[O:10])[CH2:11][C@H:12]([OH:13])[CH2:14][O:15][C:16](=[O:17])[c:18]1[cH:19][cH:20][cH:21][cH:22][cH:23]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][C@H:9]([OH:10])[CH2:11][C@H:12]([OH:13])[CH2:14][O:15][C:16](=[O:17])[c:18]1[cH:19][cH:20][cH:21...
CC(C)(C)OC(=O)CC(=O)C[C@H](O)COC(=O)c1ccccc1
CC(C)(C)OC(=O)C[C@H](O)C[C@H](O)COC(=O)c1ccccc1
null
null
P(=O)([O-])([O-])[O-]
Reduction
Reduction of ketone to secondary alcohol
02790ac194d8bf7ccb13d6247c59412024d87f77d2c906ef7804f021f57d5070
1bd3cd74b454139c0a0068ac0135836499926b274bff569df163210c6c944a89
c1ccccc1
[C:1]-[C:2]-[C;H0;D3;+0:3](=[O;H0;D1;+0:4])-[C:5]-[C:6](=[O;D1;H0:7])-[#8:8]-[C:9](-[C;D1;H3:10])(-[C;D1;H3:11])-[C;D1;H3:12]>>[C:1]-[C:2]-[C@@H;D3;+0:3](-[OH;D1;+0:4])-[C:5]-[C:6](=[O;D1;H0:7])-[#8:8]-[C:9](-[C;D1;H3:10])(-[C;D1;H3:11])-[C;D1;H3:12]
null
[]
null
null
null
null
Using 5 ml of Medium C described hereinbefore, the microorganisms indicated in Table 4 were cultured in the same manner as in Example 11. From 5 ml of each culture, the cells were centrifugally harvested, suspended in 0.5 ml of 100 mM phosphate buffer (pH 6.5) containing 0.05% of (5S)-6-benzoyloxy-5-hydroxy-3-oxohexano...
10.6084/m9.figshare.5104873.v1
null
Ketone
Secondary alcohol
null
null
c1ccccc1
null
P(=O)([O-])([O-])[O-]
null
null
CC(C)(C)OC(=O)CC(=O)C[C@H](O)COC(=O)c1ccccc1>P(=O)([O-])([O-])[O-]>CC(C)(C)OC(=O)C[C@H](O)C[C@H](O)COC(=O)c1ccccc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-980177fca8a041c8ab1d3755eefdece6
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(C)(C)OC>>CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
C(O)([O-])=O.[Na+].C(C)(C)(C)OC(CC(C[C@@H](COC(C1=CC=CC=C1)=O)O)O)=O.COC(C)(C)OC>>C(C)(C)(C)OC(C[C@@H]1OC(O[C@@H](C1)COC(C1=CC=CC=C1)=O)(C)C)=O
[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][CH:9]([CH2:10][C@@H:11]([CH2:12][O:13][C:14](=[O:15])[c:16]1[cH:17][cH:18][cH:19][cH:20][cH:21]1)[OH:22])[OH:26].CO[C:23](OC)([CH3:24])[CH3:25]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][C@H:9]1[CH2:10][C@@H:11]([CH2:12][O:13][C:14](=[O:15])[c:16]2[c...
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(C)(C)OC
CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
null
null
C(Cl)Cl
Heteroatom Alkylation and Arylation
OtherReaction
1b897a1df0e5845a2b8f88001414f79fb5194fee7b162720b2a7cd50dadd1aa0
5b3ed0191ba86b6e1048e761d184b2389fdc2075f66c7c9aaba67c74a6cbc43e
O=C(OC[C@@H]1CCOCO1)c1ccccc1
C-O-[C;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-O-C.[C:4]-[C:5](-[OH;D1;+0:6])-[C:7]-[CH;D3;+0:8](-[OH;D1;+0:9])-[C:10]-[C:11](=[O;D1;H0:12])-[#8:13]-[C:14](-[C;D1;H3:15])(-[C;D1;H3:16])-[C;D1;H3:17]>>[C:4]-[C:5]1-[C:7]-[C@H;D3;+0:8](-[C:10]-[C:11](=[O;D1;H0:12])-[#8:13]-[C:14](-[C;D1;H3:15])(-[C;D1;H3:16])-[C;D1;H3:17]...
72
[{"value": 72.0, "product": "C(C)(C)(C)OC(C[C@@H]1OC(O[C@@H](C1)COC(C1=CC=CC=C1)=O)(C)C)=O", "details": "PERCENTYIELD", "is_desired": false}]
20
CELSIUS
4
HOUR
To a solution composed of 8.94 g (27.6 mmol) of (5S)-6-benzoyloxy-3,5-dihydroxyhexanoic tert-butyl ester produced in Example 15, 35.8 mL of 2,2-dimethoxypropane, and 2.5 mL of methylene chloride was added 269 mg (1.4 mmol) of p-toluenesulfonic acid-1H2O, and the mixture was stirred at 20° C. for 4 hours, after which 50...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Secondary alcohol.Secondary alcohol
Ether.Ether
null
C1COCOC1
C1COCOC1.c1ccccc1
HO-
C(Cl)Cl
20
4
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(C)(C)OC>C(Cl)Cl>CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-4a04649c10df4184a5d8aa78ef30e2a3
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(C)(C)OC>>CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
C1(=CC=C(C=C1)S(=O)(=O)O)C.C(C)(C)(C)OC(CC(C[C@@H](COC(C1=CC=CC=C1)=O)O)O)=O.COC(C)(C)OC.CC(=O)C>>C(C)(C)(C)OC(C[C@@H]1OC(O[C@@H](C1)COC(C1=CC=CC=C1)=O)(C)C)=O
[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][CH:9]([CH2:10][C@@H:11]([CH2:12][O:13][C:14](=[O:15])[c:16]1[cH:17][cH:18][cH:19][cH:20][cH:21]1)[OH:22])[OH:26].CO[C:23](OC)([CH3:24])[CH3:25]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][C@H:9]1[CH2:10][C@@H:11]([CH2:12][O:13][C:14](=[O:15])[c:16]2[c...
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(C)(C)OC
CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
null
null
O.C(C)#N
Heteroatom Alkylation and Arylation
OtherReaction
1b897a1df0e5845a2b8f88001414f79fb5194fee7b162720b2a7cd50dadd1aa0
5b3ed0191ba86b6e1048e761d184b2389fdc2075f66c7c9aaba67c74a6cbc43e
O=C(OC[C@@H]1CCOCO1)c1ccccc1
C-O-[C;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-O-C.[C:4]-[C:5](-[OH;D1;+0:6])-[C:7]-[CH;D3;+0:8](-[OH;D1;+0:9])-[C:10]-[C:11](=[O;D1;H0:12])-[#8:13]-[C:14](-[C;D1;H3:15])(-[C;D1;H3:16])-[C;D1;H3:17]>>[C:4]-[C:5]1-[C:7]-[C@H;D3;+0:8](-[C:10]-[C:11](=[O;D1;H0:12])-[#8:13]-[C:14](-[C;D1;H3:15])(-[C;D1;H3:16])-[C;D1;H3:17]...
null
[]
40
CELSIUS
16
HOUR
To a solution composed of 108 mg (90.2 weight %, 0.3 mmol) of the (5S)-6-benzoyloxy-3,5-dihydroxyhexanoic tert-butyl ester produced in Example 15, 62.4 mg (0.6 mmol) of 2,2-dimethoxypropane, and 5 mL of acetone was added 5.7 mg (0.03 mmol) of p-toluenesulfonic acid.1H2O, and the mixture was stirred at 40° C. for 16 hou...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Secondary alcohol.Secondary alcohol
Ether.Ether
null
C1COCOC1
C1COCOC1.c1ccccc1
HO-
O.C(C)#N
40
16
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(C)(C)OC>O.C(C)#N>CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-0993d93248bf475d918c0a23581a47a7
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1>>CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
C(C)(C)(C)OC(CC(C[C@@H](COC(C1=CC=CC=C1)=O)O)O)=O.O[C@@H]1C[C@H](OC(C1)=O)COC(C1=CC=CC=C1)=O.COC(C[C@@H]1OC(O[C@@H](C1)COC(C1=CC=CC=C1)=O)(C)C)=O>>C(C)(C)(C)OC(C[C@@H]1OC(O[C@@H](C1)COC(C1=CC=CC=C1)=O)(C)C)=O
O=C(OC[C@@H](O)CC(O)[CH2:8][C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])c1ccccc1.COC(=O)C[C@H:9]1[CH2:10][C@@H:11]([CH2:12][O:13][C:14](=[O:15])[c:16]2[cH:17][cH:18][cH:19][cH:20][cH:21]2)[O:22][C:23]([CH3:24])([CH3:25])[O:26]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][C@H:9]1[CH2:10][C@@H:11]([CH2:1...
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
null
null
null
C-C Coupling
OtherReaction
c60ef6ec5a2c9d314090af95d014b97611eb1c633b6c4edd79357c82b20f8fda
eae68fb503126ff52b24216efa23df03bfbd9669bc67803b9ac2cd9653b8c829
O=C(OC[C@@H]1CCOCO1)c1ccccc1
C-O-C(=O)-C-[C@@H;D3;+0:1]1-[#8:2]-[C:3]-[#8:4]-[C:5]-[C:6]-1.O-C(-C-[C@@H](-O)-C-O-C(=O)-c1:c:c:c:c:c:1)-[CH2;D2;+0:7]-[C:8](=[O;D1;H0:9])-[#8:10]-[C:11](-[C;D1;H3:12])(-[C;D1;H3:13])-[C;D1;H3:14]>>[C;D1;H3:12]-[C:11](-[C;D1;H3:13])(-[C;D1;H3:14])-[#8:10]-[C:8](=[O;D1;H0:9])-[CH2;D2;+0:7]-[C@@H;D3;+0:1]1-[#8:2]-[C:3]-...
null
[]
null
null
null
null
78.8%; (5S)-6-benzoyloxy-3,5-dihydroxyhexanoic tert-butyl ester: 7.5%; (2S,4R)-4-hydroxy-6-oxo-2-[(benzoyloxy)methyl]tetrahydro-2H-pyran: 5.9%; 2-[(4R,6S)-2,2-dimethyl-6-benzoyloxymethyl-1,3-dioxan-4-yl]acetic methyl ester: 3.0%. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Ester.Ester.Ester.Ether.Secondary alcohol.Secondary alcohol
Ester.Ether
c1ccccc1.C1COCOC1
C1COCOC1
C1COCOC1.c1ccccc1
HO-
null
null
null
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1>>CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-b6dcf5cdee5f4580990d89ae67e88dda
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(C)(C)OC>>CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
N1=CC=CC=C1.C(C)(C)(C)OC(CC(C[C@@H](COC(C1=CC=CC=C1)=O)O)O)=O.COC(C)(C)OC.C1(=CC=C(C=C1)S(=O)(=O)O)C>>C(C)(C)(C)OC(C[C@@H]1OC(O[C@@H](C1)COC(C1=CC=CC=C1)=O)(C)C)=O
[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][CH:9]([CH2:10][C@@H:11]([CH2:12][O:13][C:14](=[O:15])[c:16]1[cH:17][cH:18][cH:19][cH:20][cH:21]1)[OH:22])[OH:26].CO[C:23](OC)([CH3:24])[CH3:25]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][C@H:9]1[CH2:10][C@@H:11]([CH2:12][O:13][C:14](=[O:15])[c:16]2[c...
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(C)(C)OC
CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
null
null
CC(=O)C.O.C(C)#N
Heteroatom Alkylation and Arylation
OtherReaction
1b897a1df0e5845a2b8f88001414f79fb5194fee7b162720b2a7cd50dadd1aa0
5b3ed0191ba86b6e1048e761d184b2389fdc2075f66c7c9aaba67c74a6cbc43e
O=C(OC[C@@H]1CCOCO1)c1ccccc1
C-O-[C;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-O-C.[C:4]-[C:5](-[OH;D1;+0:6])-[C:7]-[CH;D3;+0:8](-[OH;D1;+0:9])-[C:10]-[C:11](=[O;D1;H0:12])-[#8:13]-[C:14](-[C;D1;H3:15])(-[C;D1;H3:16])-[C;D1;H3:17]>>[C:4]-[C:5]1-[C:7]-[C@H;D3;+0:8](-[C:10]-[C:11](=[O;D1;H0:12])-[#8:13]-[C:14](-[C;D1;H3:15])(-[C;D1;H3:16])-[C;D1;H3:17]...
null
[]
null
null
null
null
To a solution composed of 108 mg (90.2 weight %, 0.3 mmol) of the (5S)-6-benzoyloxy-3,5-dihydroxyhexanoic tert-butyl ester produced in Example 15, 62.4 mg (0.6 mmol) of 2,2-dimethoxypropane, and 5 mL of acetone were added 5.7 mg (0.03 mmol) of p-toluenesulfonic acid.1H2O and 11.9 mg (0.15 mmol) of pyridine, and the mix...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Secondary alcohol.Secondary alcohol
Ether.Ether
null
C1COCOC1
C1COCOC1.c1ccccc1
HO-
CC(=O)C.O.C(C)#N
null
null
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(C)(C)OC>CC(=O)C.O.C(C)#N>CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-b8e538f0579c41db942698431874f3f6
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1>>CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
C(C)(C)(C)OC(CC(C[C@@H](COC(C1=CC=CC=C1)=O)O)O)=O.O[C@@H]1C[C@H](OC(C1)=O)COC(C1=CC=CC=C1)=O.COC(C[C@@H]1OC(O[C@@H](C1)COC(C1=CC=CC=C1)=O)(C)C)=O>>C(C)(C)(C)OC(C[C@@H]1OC(O[C@@H](C1)COC(C1=CC=CC=C1)=O)(C)C)=O
O=C(OC[C@@H](O)CC(O)[CH2:8][C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])c1ccccc1.COC(=O)C[C@H:9]1[CH2:10][C@@H:11]([CH2:12][O:13][C:14](=[O:15])[c:16]2[cH:17][cH:18][cH:19][cH:20][cH:21]2)[O:22][C:23]([CH3:24])([CH3:25])[O:26]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][C@H:9]1[CH2:10][C@@H:11]([CH2:1...
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
null
null
null
C-C Coupling
OtherReaction
c60ef6ec5a2c9d314090af95d014b97611eb1c633b6c4edd79357c82b20f8fda
eae68fb503126ff52b24216efa23df03bfbd9669bc67803b9ac2cd9653b8c829
O=C(OC[C@@H]1CCOCO1)c1ccccc1
C-O-C(=O)-C-[C@@H;D3;+0:1]1-[#8:2]-[C:3]-[#8:4]-[C:5]-[C:6]-1.O-C(-C-[C@@H](-O)-C-O-C(=O)-c1:c:c:c:c:c:1)-[CH2;D2;+0:7]-[C:8](=[O;D1;H0:9])-[#8:10]-[C:11](-[C;D1;H3:12])(-[C;D1;H3:13])-[C;D1;H3:14]>>[C;D1;H3:12]-[C:11](-[C;D1;H3:13])(-[C;D1;H3:14])-[#8:10]-[C:8](=[O;D1;H0:9])-[CH2;D2;+0:7]-[C@@H;D3;+0:1]1-[#8:2]-[C:3]-...
null
[]
null
null
null
null
93.1%; (5S)-6-benzoyloxy-3,5-dihydroxyhexanoic tert-butyl ester: 3.4%; (2S,4R)-4-hydroxy-6-oxo-2-[(benzoyloxy)methyl]tetrahydro-2H-pyran: 0.1%; 2-[(4R,6S)-2,2-dimethyl-6-benzoyloxymethyl-1,3-dioxan-4-yl]acetic methyl ester: 0.1%. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Ester.Ester.Ester.Ether.Secondary alcohol.Secondary alcohol
Ester.Ether
c1ccccc1.C1COCOC1
C1COCOC1
C1COCOC1.c1ccccc1
HO-
null
null
null
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1>>CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-24353d021c514b1880414b4e363889fe
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(C)(C)OC>>CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
C(C)N(CC)CC.C(C)(C)(C)OC(CC(C[C@@H](COC(C1=CC=CC=C1)=O)O)O)=O.COC(C)(C)OC.C1(=CC=C(C=C1)S(=O)(=O)O)C>>C(C)(C)(C)OC(C[C@@H]1OC(O[C@@H](C1)COC(C1=CC=CC=C1)=O)(C)C)=O
[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][CH:9]([CH2:10][C@@H:11]([CH2:12][O:13][C:14](=[O:15])[c:16]1[cH:17][cH:18][cH:19][cH:20][cH:21]1)[OH:22])[OH:26].CO[C:23](OC)([CH3:24])[CH3:25]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][C@H:9]1[CH2:10][C@@H:11]([CH2:12][O:13][C:14](=[O:15])[c:16]2[c...
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(C)(C)OC
CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
null
null
CC(=O)C.O.C(C)#N
Heteroatom Alkylation and Arylation
OtherReaction
1b897a1df0e5845a2b8f88001414f79fb5194fee7b162720b2a7cd50dadd1aa0
5b3ed0191ba86b6e1048e761d184b2389fdc2075f66c7c9aaba67c74a6cbc43e
O=C(OC[C@@H]1CCOCO1)c1ccccc1
C-O-[C;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-O-C.[C:4]-[C:5](-[OH;D1;+0:6])-[C:7]-[CH;D3;+0:8](-[OH;D1;+0:9])-[C:10]-[C:11](=[O;D1;H0:12])-[#8:13]-[C:14](-[C;D1;H3:15])(-[C;D1;H3:16])-[C;D1;H3:17]>>[C:4]-[C:5]1-[C:7]-[C@H;D3;+0:8](-[C:10]-[C:11](=[O;D1;H0:12])-[#8:13]-[C:14](-[C;D1;H3:15])(-[C;D1;H3:16])-[C;D1;H3:17]...
null
[]
null
null
null
null
To a solution composed of 108 mg (90.2 weight %, 0.3 mmol) of the (5S)-6-benzoyloxy-3,5-dihydroxyhexanoic tert-butyl ester produced in Example 15, 62.4 mg (0.6 mmol) of 2,2-dimethoxypropane, and 5 mL of acetone were added 5.7 mg (0.03 mmol) of p-toluenesulfonic acid.1H2O and 15.2 mg (0.15 mmol) of triethylamine, and th...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Secondary alcohol.Secondary alcohol
Ether.Ether
null
C1COCOC1
C1COCOC1.c1ccccc1
HO-
CC(=O)C.O.C(C)#N
null
null
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(C)(C)OC>CC(=O)C.O.C(C)#N>CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-bdf8bb4b2ddc49f28298a435bb43b722
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1>>CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
C(C)(C)(C)OC(CC(C[C@@H](COC(C1=CC=CC=C1)=O)O)O)=O.O[C@@H]1C[C@H](OC(C1)=O)COC(C1=CC=CC=C1)=O.COC(C[C@@H]1OC(O[C@@H](C1)COC(C1=CC=CC=C1)=O)(C)C)=O>>C(C)(C)(C)OC(C[C@@H]1OC(O[C@@H](C1)COC(C1=CC=CC=C1)=O)(C)C)=O
O=C(OC[C@@H](O)CC(O)[CH2:8][C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])c1ccccc1.COC(=O)C[C@H:9]1[CH2:10][C@@H:11]([CH2:12][O:13][C:14](=[O:15])[c:16]2[cH:17][cH:18][cH:19][cH:20][cH:21]2)[O:22][C:23]([CH3:24])([CH3:25])[O:26]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][C@H:9]1[CH2:10][C@@H:11]([CH2:1...
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
null
null
null
C-C Coupling
OtherReaction
c60ef6ec5a2c9d314090af95d014b97611eb1c633b6c4edd79357c82b20f8fda
eae68fb503126ff52b24216efa23df03bfbd9669bc67803b9ac2cd9653b8c829
O=C(OC[C@@H]1CCOCO1)c1ccccc1
C-O-C(=O)-C-[C@@H;D3;+0:1]1-[#8:2]-[C:3]-[#8:4]-[C:5]-[C:6]-1.O-C(-C-[C@@H](-O)-C-O-C(=O)-c1:c:c:c:c:c:1)-[CH2;D2;+0:7]-[C:8](=[O;D1;H0:9])-[#8:10]-[C:11](-[C;D1;H3:12])(-[C;D1;H3:13])-[C;D1;H3:14]>>[C;D1;H3:12]-[C:11](-[C;D1;H3:13])(-[C;D1;H3:14])-[#8:10]-[C:8](=[O;D1;H0:9])-[CH2;D2;+0:7]-[C@@H;D3;+0:1]1-[#8:2]-[C:3]-...
null
[]
null
null
null
null
93.3%; (5S)-6-benzoyloxy-3,5-dihydroxyhexanoic tert-butyl ester: 3.0%; (2S, 4R)-4-hydroxy-6-oxo-2-[(benzoyloxy)methyl]tetrahydro-2H-pyran: 0.1%; 2-[(4R, 6S)-2,2-dimethyl-6-benzoyloxymethyl-1,3-dioxan-4-yl]acetic methyl ester: 0.1%. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Ester.Ester.Ester.Ether.Secondary alcohol.Secondary alcohol
Ester.Ether
c1ccccc1.C1COCOC1
C1COCOC1
C1COCOC1.c1ccccc1
HO-
null
null
null
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1>>CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-1166148f5b4d48509429004f74eb2ee2
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(C)(C)OC>>CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
N1C=NC=C1.C(C)(C)(C)OC(CC(C[C@@H](COC(C1=CC=CC=C1)=O)O)O)=O.COC(C)(C)OC.C1(=CC=C(C=C1)S(=O)(=O)O)C>>C(C)(C)(C)OC(C[C@@H]1OC(O[C@@H](C1)COC(C1=CC=CC=C1)=O)(C)C)=O
[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][CH:9]([CH2:10][C@@H:11]([CH2:12][O:13][C:14](=[O:15])[c:16]1[cH:17][cH:18][cH:19][cH:20][cH:21]1)[OH:22])[OH:26].CO[C:23](OC)([CH3:24])[CH3:25]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][C@H:9]1[CH2:10][C@@H:11]([CH2:12][O:13][C:14](=[O:15])[c:16]2[c...
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(C)(C)OC
CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
null
null
CC(=O)C.O.C(C)#N
Heteroatom Alkylation and Arylation
OtherReaction
1b897a1df0e5845a2b8f88001414f79fb5194fee7b162720b2a7cd50dadd1aa0
5b3ed0191ba86b6e1048e761d184b2389fdc2075f66c7c9aaba67c74a6cbc43e
O=C(OC[C@@H]1CCOCO1)c1ccccc1
C-O-[C;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-O-C.[C:4]-[C:5](-[OH;D1;+0:6])-[C:7]-[CH;D3;+0:8](-[OH;D1;+0:9])-[C:10]-[C:11](=[O;D1;H0:12])-[#8:13]-[C:14](-[C;D1;H3:15])(-[C;D1;H3:16])-[C;D1;H3:17]>>[C:4]-[C:5]1-[C:7]-[C@H;D3;+0:8](-[C:10]-[C:11](=[O;D1;H0:12])-[#8:13]-[C:14](-[C;D1;H3:15])(-[C;D1;H3:16])-[C;D1;H3:17]...
null
[]
null
null
null
null
To a solution composed of 108 mg (90.2 weight %, 0.3 mmol) of the (5S)-6-benzoyloxy-3,5-dihydroxyhexanoic tert-butyl ester produced in Example 15, 62.4 mg (0.6 mmol) of 2,2-dimethoxypropane, and 5 mL of acetone were added 5.7 mg (0.03 mmol) of p-toluenesulfonic acid.1H2O and 10.2 mg (0.15 mmol) of imidazole, and the mi...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Secondary alcohol.Secondary alcohol
Ether.Ether
null
C1COCOC1
C1COCOC1.c1ccccc1
HO-
CC(=O)C.O.C(C)#N
null
null
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(C)(C)OC>CC(=O)C.O.C(C)#N>CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-6bd7853f654c47c781dcb1430a6b6a20
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1>>CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
C(C)(C)(C)OC(CC(C[C@@H](COC(C1=CC=CC=C1)=O)O)O)=O.O[C@@H]1C[C@H](OC(C1)=O)COC(C1=CC=CC=C1)=O.COC(C[C@@H]1OC(O[C@@H](C1)COC(C1=CC=CC=C1)=O)(C)C)=O>>C(C)(C)(C)OC(C[C@@H]1OC(O[C@@H](C1)COC(C1=CC=CC=C1)=O)(C)C)=O
O=C(OC[C@@H](O)CC(O)[CH2:8][C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])c1ccccc1.COC(=O)C[C@H:9]1[CH2:10][C@@H:11]([CH2:12][O:13][C:14](=[O:15])[c:16]2[cH:17][cH:18][cH:19][cH:20][cH:21]2)[O:22][C:23]([CH3:24])([CH3:25])[O:26]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][C@H:9]1[CH2:10][C@@H:11]([CH2:1...
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
null
null
null
C-C Coupling
OtherReaction
c60ef6ec5a2c9d314090af95d014b97611eb1c633b6c4edd79357c82b20f8fda
eae68fb503126ff52b24216efa23df03bfbd9669bc67803b9ac2cd9653b8c829
O=C(OC[C@@H]1CCOCO1)c1ccccc1
C-O-C(=O)-C-[C@@H;D3;+0:1]1-[#8:2]-[C:3]-[#8:4]-[C:5]-[C:6]-1.O-C(-C-[C@@H](-O)-C-O-C(=O)-c1:c:c:c:c:c:1)-[CH2;D2;+0:7]-[C:8](=[O;D1;H0:9])-[#8:10]-[C:11](-[C;D1;H3:12])(-[C;D1;H3:13])-[C;D1;H3:14]>>[C;D1;H3:12]-[C:11](-[C;D1;H3:13])(-[C;D1;H3:14])-[#8:10]-[C:8](=[O;D1;H0:9])-[CH2;D2;+0:7]-[C@@H;D3;+0:1]1-[#8:2]-[C:3]-...
null
[]
null
null
null
null
93.9%; (5S)-6-benzoyloxy-3,5-dihydroxyhexanoic tert-butyl ester: 3.0%; (2S,4R)-4-hydroxy-6-oxo-2-[(benzoyloxy)methyl]tetrahydro-2H-pyran: 0.1%; 2-[(4R,6S)-2,2-dimethyl-6-benzoyloxymethyl-1,3-dioxan-4-yl]acetic methyl ester: 0.1%. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Ester.Ester.Ester.Ether.Secondary alcohol.Secondary alcohol
Ester.Ether
c1ccccc1.C1COCOC1
C1COCOC1
C1COCOC1.c1ccccc1
HO-
null
null
null
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1>>CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-d475ed245f9540058b93905df4149af0
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(C)(C)OC>>CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
CC=1C=NC=CC1.C(C)(C)(C)OC(CC(C[C@@H](COC(C1=CC=CC=C1)=O)O)O)=O.COC(C)(C)OC.C1(=CC=C(C=C1)S(=O)(=O)O)C>>C(C)(C)(C)OC(C[C@@H]1OC(O[C@@H](C1)COC(C1=CC=CC=C1)=O)(C)C)=O
[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][CH:9]([CH2:10][C@@H:11]([CH2:12][O:13][C:14](=[O:15])[c:16]1[cH:17][cH:18][cH:19][cH:20][cH:21]1)[OH:22])[OH:26].CO[C:23](OC)([CH3:24])[CH3:25]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][C@H:9]1[CH2:10][C@@H:11]([CH2:12][O:13][C:14](=[O:15])[c:16]2[c...
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(C)(C)OC
CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
null
null
CC(=O)C.O.C(C)#N
Heteroatom Alkylation and Arylation
OtherReaction
1b897a1df0e5845a2b8f88001414f79fb5194fee7b162720b2a7cd50dadd1aa0
5b3ed0191ba86b6e1048e761d184b2389fdc2075f66c7c9aaba67c74a6cbc43e
O=C(OC[C@@H]1CCOCO1)c1ccccc1
C-O-[C;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-O-C.[C:4]-[C:5](-[OH;D1;+0:6])-[C:7]-[CH;D3;+0:8](-[OH;D1;+0:9])-[C:10]-[C:11](=[O;D1;H0:12])-[#8:13]-[C:14](-[C;D1;H3:15])(-[C;D1;H3:16])-[C;D1;H3:17]>>[C:4]-[C:5]1-[C:7]-[C@H;D3;+0:8](-[C:10]-[C:11](=[O;D1;H0:12])-[#8:13]-[C:14](-[C;D1;H3:15])(-[C;D1;H3:16])-[C;D1;H3:17]...
null
[]
null
null
null
null
To a solution composed of 108 mg (90.2 weight %, 0.3 mmol) of the (5S)-6-benzoyloxy-3,5-dihydroxyhexanoic tert-butyl ester produced in Example 15, 62.4 mg (0.6 mmol) of 2,2-dimethoxypropane, and 5 mL of acetone were added 5.7 mg (0.03 mmol) of p-toluenesulfonic acid.1H2O and 14.0 mg (0.15 mmol) of 3-methylpyridine, and...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Secondary alcohol.Secondary alcohol
Ether.Ether
null
C1COCOC1
C1COCOC1.c1ccccc1
HO-
CC(=O)C.O.C(C)#N
null
null
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(C)(C)OC>CC(=O)C.O.C(C)#N>CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-76b1b6cdfdab46429b9b29b828b67971
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1>>CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
C(C)(C)(C)OC(CC(C[C@@H](COC(C1=CC=CC=C1)=O)O)O)=O.O[C@@H]1C[C@H](OC(C1)=O)COC(C1=CC=CC=C1)=O.COC(C[C@@H]1OC(O[C@@H](C1)COC(C1=CC=CC=C1)=O)(C)C)=O>>C(C)(C)(C)OC(C[C@@H]1OC(O[C@@H](C1)COC(C1=CC=CC=C1)=O)(C)C)=O
O=C(OC[C@@H](O)CC(O)[CH2:8][C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])c1ccccc1.COC(=O)C[C@H:9]1[CH2:10][C@@H:11]([CH2:12][O:13][C:14](=[O:15])[c:16]2[cH:17][cH:18][cH:19][cH:20][cH:21]2)[O:22][C:23]([CH3:24])([CH3:25])[O:26]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][C@H:9]1[CH2:10][C@@H:11]([CH2:1...
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1
null
null
null
C-C Coupling
OtherReaction
c60ef6ec5a2c9d314090af95d014b97611eb1c633b6c4edd79357c82b20f8fda
eae68fb503126ff52b24216efa23df03bfbd9669bc67803b9ac2cd9653b8c829
O=C(OC[C@@H]1CCOCO1)c1ccccc1
C-O-C(=O)-C-[C@@H;D3;+0:1]1-[#8:2]-[C:3]-[#8:4]-[C:5]-[C:6]-1.O-C(-C-[C@@H](-O)-C-O-C(=O)-c1:c:c:c:c:c:1)-[CH2;D2;+0:7]-[C:8](=[O;D1;H0:9])-[#8:10]-[C:11](-[C;D1;H3:12])(-[C;D1;H3:13])-[C;D1;H3:14]>>[C;D1;H3:12]-[C:11](-[C;D1;H3:13])(-[C;D1;H3:14])-[#8:10]-[C:8](=[O;D1;H0:9])-[CH2;D2;+0:7]-[C@@H;D3;+0:1]1-[#8:2]-[C:3]-...
null
[]
null
null
null
null
93.8%; (5S)-6-benzoyloxy-3,5-dihydroxyhexanoic tert-butyl ester: 2.8%; (2S,4R)-4-hydroxy-6-oxo-2-[(benzoyloxy)methyl]tetrahydro-2H-pyran: 0.1%; 2-[(4R,6S)-2,2-dimethyl-6-benzoyloxymethyl-1,3-dioxan-4-yl]acetic methyl ester: 0.1%. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Ester.Ester.Ester.Ether.Secondary alcohol.Secondary alcohol
Ester.Ether
c1ccccc1.C1COCOC1
C1COCOC1
C1COCOC1.c1ccccc1
HO-
null
null
null
CC(C)(C)OC(=O)CC(O)C[C@H](O)COC(=O)c1ccccc1.COC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1>>CC(C)(C)OC(=O)C[C@H]1C[C@@H](COC(=O)c2ccccc2)OC(C)(C)O1