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large_stringclasses
414 values
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large_stringlengths
36
36
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large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
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14
3.37k
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large_stringlengths
1
581
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large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
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float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
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large_stringclasses
3 values
reaction_time_value
float64
0
4k
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large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e620bb8c96c044ae89795f40aff01e3e
CCOC(=O)c1c[nH]c(-c2ccccc2)c1>>OCc1c[nH]c(-c2ccccc2)c1
O.[H-].C(C(C)C)[Al+]CC(C)C.C1(=CC=CC=C1)C1=CC(=CN1)C(=O)OCC>>C1(=CC=CC=C1)C1=CC(=CN1)CO
CCO[C:2](=[O:1])[c:3]1[cH:4][nH:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][cH:11][cH:12]2)[cH:13]1>>[OH:1][CH2:2][c:3]1[cH:4][nH:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][cH:11][cH:12]2)[cH:13]1
CCOC(=O)c1c[nH]c(-c2ccccc2)c1
OCc1c[nH]c(-c2ccccc2)c1
null
null
O1CCCC1.C1(=CC=CC=C1)C
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
c1ccc(-c2ccc[nH]2)cc1
C-C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[c:7]:1>>[OH;D1;+0:2]-[CH2;D2;+0:1]-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[c:7]:1
87
[{"value": 87.0, "product": "C1(=CC=CC=C1)C1=CC(=CN1)CO", "details": "PERCENTYIELD", "is_desired": false}, {"value": 86.9, "product": "C1(=CC=CC=C1)C1=CC(=CN1)CO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-78
CELSIUS
1
HOUR
A solution (100 mL) of ethyl 5-phenyl-1H-pyrrole-3-carboxylate (2.16 g) in tetrahydrofuran was cooled to −78° C., and a 1.5 mol/L solution (24 mL) of diisobutylaluminum hydride in toluene was added dropwise over 10 min. The mixture was further stirred at −78° C. for 1 hr, water (2 mL) was added dropwise over 2 min, and...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
c1cc[nH]c1.c1ccccc1
HO-
O1CCCC1.C1(=CC=CC=C1)C
-78
1
CCOC(=O)c1c[nH]c(-c2ccccc2)c1>O1CCCC1.C1(=CC=CC=C1)C>OCc1c[nH]c(-c2ccccc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ff64cf2715224e8988e69887cb80030a
OCc1c[nH]c(-c2ccccc2)c1>>O=Cc1c[nH]c(-c2ccccc2)c1
C1(=CC=CC=C1)C1=CC(=CN1)CO.C[N+]1(CCOCC1)[O-]>>C1(=CC=CC=C1)C1=CC(=CN1)C=O
[OH:1][CH2:2][c:3]1[cH:4][nH:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][cH:11][cH:12]2)[cH:13]1>>[O:1]=[CH:2][c:3]1[cH:4][nH:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][cH:11][cH:12]2)[cH:13]1
OCc1c[nH]c(-c2ccccc2)c1
O=Cc1c[nH]c(-c2ccccc2)c1
null
[Ru](=O)(=O)(=O)[O-].C(CC)[N+](CCC)(CCC)CCC
C(C)#N
Oxidation
Oxidation or Dehydrogenation of Alcohols to Aldehydes and Ketones
41bfa9deea81b465c88ad21fdfb64a2e1ba29490558cf430df132cb98b4a538b
0a03c6724c1862e8f86d4a463afda55b8e067dc6cb42597b472eb7cabc03eda3
c1ccc(-c2ccc[nH]2)cc1
[OH;D1;+0:1]-[CH2;D2;+0:2]-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[c:7]:1>>[O;H0;D1;+0:1]=[CH;D2;+0:2]-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[c:7]:1
62
[{"value": 62.0, "product": "C1(=CC=CC=C1)C1=CC(=CN1)C=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 61.6, "product": "C1(=CC=CC=C1)C1=CC(=CN1)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1.5
HOUR
To a solution (45 mL) of (5-phenyl-1H-pyrrol-3-yl)methanol (1.51 g) in acetonitrile were added tetra-n-propylammonium perruthenate (0.46 g), N-methylmorpholine N-oxide (2.36 g) and molecular sieves 4A powder (4.5 g), and the mixture was stirred at room temperature for 1.5 hr. The reaction mixture was filtered through c...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Aldehyde
null
null
c1cc[nH]c1.c1ccccc1
null
[Ru](=O)(=O)(=O)[O-].C(CC)[N+](CCC)(CCC)CCC.C(C)#N
null
1.5
OCc1c[nH]c(-c2ccccc2)c1>[Ru](=O)(=O)(=O)[O-].C(CC)[N+](CCC)(CCC)CCC.C(C)#N>O=Cc1c[nH]c(-c2ccccc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-263eb300394041fc896f191d181331c3
Cc1c(CO)c[nH]c1-c1ccccc1F>>Cc1c(C=O)c[nH]c1-c1ccccc1F
FC1=C(C=CC=C1)C1=C(C(=CN1)CO)C.C[N+]1(CCOCC1)[O-]>>FC1=C(C=CC=C1)C1=C(C(=CN1)C=O)C
[CH3:1][c:2]1[c:3]([CH2:4][OH:5])[cH:6][nH:7][c:8]1-[c:9]1[cH:10][cH:11][cH:12][cH:13][c:14]1[F:15]>>[CH3:1][c:2]1[c:3]([CH:4]=[O:5])[cH:6][nH:7][c:8]1-[c:9]1[cH:10][cH:11][cH:12][cH:13][c:14]1[F:15]
Cc1c(CO)c[nH]c1-c1ccccc1F
Cc1c(C=O)c[nH]c1-c1ccccc1F
null
[Ru](=O)(=O)(=O)[O-].C(CC)[N+](CCC)(CCC)CCC
null
Oxidation
Oxidation or Dehydrogenation of Alcohols to Aldehydes and Ketones
41bfa9deea81b465c88ad21fdfb64a2e1ba29490558cf430df132cb98b4a538b
0a03c6724c1862e8f86d4a463afda55b8e067dc6cb42597b472eb7cabc03eda3
c1ccc(-c2ccc[nH]2)cc1
[OH;D1;+0:1]-[CH2;D2;+0:2]-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[c:7]:1>>[O;H0;D1;+0:1]=[CH;D2;+0:2]-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[c:7]:1
58
[{"value": 58.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a similar operation as in Reference Example 15 and using [5-(2-fluorophenyl)-4-methyl-1H-pyrrol-3-yl]methanol (1.17 g), tetra-n-propylammonium perruthenate (101 mg), N-methylmorpholine N-oxide (1.01 g) and molecular sieves 4A powder (572 mg), the title compound was obtained as pale-pink crystals (yield 0.67 g, 58%)....
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Aldehyde
null
null
c1cc[nH]c1.c1ccccc1
null
[Ru](=O)(=O)(=O)[O-].C(CC)[N+](CCC)(CCC)CCC
null
null
Cc1c(CO)c[nH]c1-c1ccccc1F>[Ru](=O)(=O)(=O)[O-].C(CC)[N+](CCC)(CCC)CCC>Cc1c(C=O)c[nH]c1-c1ccccc1F
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-17120af9b4a04753ad993beb7837ed9f
C=CC(=O)OC.[C-]#[N+]CS(=O)(=O)c1ccc(C)cc1>>COC(=O)c1cc[nH]c1
O.C1(=CC=C(C=C1)S(=O)(=O)C[N+]#[C-])C.C(C=C)(=O)OC.CC(C)([O-])C.[K+]>>N1C=C(C=C1)C(=O)OC
[CH3:1][O:2][C:3](=[O:4])[CH:5]=[CH2:6].Cc1ccc(S(=O)(=O)[CH2:9][N+:8]#[C-:7])cc1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][nH:8][cH:9]1
C=CC(=O)OC.[C-]#[N+]CS(=O)(=O)c1ccc(C)cc1
COC(=O)c1cc[nH]c1
null
null
O1CCCC1
Functional Group Interconversion
OtherReaction
39f0e003eef39c7768a0aede59e10369c1ebccc1bda2d76e3203ad0a59895e73
e567b76b877c19b5a87c7a266da83a842334b0d3d7ff4a9ba0538fc9f1773f7f
c1cc[nH]c1
C-c1:c:c:c(-S(=O)(=O)-[CH2;D2;+0:1]-[N+;H0;D2:2]#[C-;H0;D1:3]):c:c:1.[C;D1;H3:4]-[#8:5]-[C:6](=[O;D1;H0:7])-[CH;D2;+0:8]=[CH2;D1;+0:9]>>[C;D1;H3:4]-[#8:5]-[C:6](=[O;D1;H0:7])-[c;H0;D3;+0:8]1:[cH;D2;+0:9]:[cH;D2;+0:3]:[nH;D2;+0:2]:[cH;D2;+0:1]:1
41
[{"value": 41.0, "product": "N1C=C(C=C1)C(=O)OC", "details": "PERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a suspension of potassium tert-butoxide (17.9 g) in tetrahydrofuran (200 mL) was added dropwise a solution of p-toluenesulfonylmethyl isocyanide (25.2 g) and methyl acrylate (11.8 mL) in tetrahydrofuran (200 mL) over 30 min. The reaction mixture was stirred at room temperature for 1 hr, water was added, and the mixt...
10.6084/m9.figshare.5104873.v1
null
Tosylate.Ester.Isocyanide.Vinyl
Ester
c1ccccc1
c1cc[nH]c1
c1cc[nH]c1
TsOH.HO-
O1CCCC1
null
1
C=CC(=O)OC.[C-]#[N+]CS(=O)(=O)c1ccc(C)cc1>O1CCCC1>COC(=O)c1cc[nH]c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-65f0efdf9d5c4c9099481cd387e4cbe3
C/C=C/C(=O)OC.[C-]#[N+]CS(=O)(=O)c1ccc(C)cc1>>COC(=O)c1c[nH]cc1C
CC(C)([O-])C.[K+].C1(=CC=C(C=C1)S(=O)(=O)C[N+]#[C-])C.C(\C=C\C)(=O)OC>>CC=1C(=CNC1)C(=O)OC
[CH3:1][O:2][C:3](=[O:4])/[CH:5]=[CH:9]/[CH3:10].Cc1ccc(S(=O)(=O)[CH2:6][N+:7]#[C-:8])cc1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][nH:7][cH:8][c:9]1[CH3:10]
C/C=C/C(=O)OC.[C-]#[N+]CS(=O)(=O)c1ccc(C)cc1
COC(=O)c1c[nH]cc1C
null
null
null
Functional Group Interconversion
OtherReaction
222aa38425ebd527cae949f4f6a41b16a79f5bedc3b38d407b2efba1132a0002
2b254751295ab0c58d4be59c7dc1148a5e0af4419b8080ba37410673480117ee
c1cc[nH]c1
C-c1:c:c:c(-S(=O)(=O)-[CH2;D2;+0:1]-[N+;H0;D2:2]#[C-;H0;D1:3]):c:c:1.[C;D1;H3:4]/[CH;D2;+0:5]=[CH;D2;+0:6]/[C:7](=[O;D1;H0:8])-[#8:9]-[C;D1;H3:10]>>[C;D1;H3:4]-[c;H0;D3;+0:5]1:[cH;D2;+0:3]:[nH;D2;+0:2]:[cH;D2;+0:1]:[c;H0;D3;+0:6]:1-[C:7](=[O;D1;H0:8])-[#8:9]-[C;D1;H3:10]
25
[{"value": 25.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a similar operation as in Reference Example 19 and using p-toluenesulfonylmethyl isocyanide (94.6 g), methyl crotonate (48.5 g) and potassium tert-butoxide (76.7 g), the title compound was obtained as a pale-yellow solid (yield 16.8 g, 25%). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Tosylate.Ester.Isocyanide
Ester
c1ccccc1
c1cc[nH]c1
c1cc[nH]c1
TsOH.HO-
null
null
null
C/C=C/C(=O)OC.[C-]#[N+]CS(=O)(=O)c1ccc(C)cc1>>COC(=O)c1c[nH]cc1C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8906695c0511400ab6aa653e9d58e236
C=COC(C)=O.CCOC(=O)CC(C)=O.N>>CCOC(=O)c1cc[nH]c1C
N.C(C)(=O)OC=C.BrBr.O=C(CC(=O)OCC)C>>CC=1NC=CC1C(=O)OCC
CC(=O)O[CH:8]=[CH2:7].O=[C:10]([CH2:6][C:4]([O:3][CH2:2][CH3:1])=[O:5])[CH3:11].[NH3:9]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][nH:9][c:10]1[CH3:11]
C=COC(C)=O.CCOC(=O)CC(C)=O.N
CCOC(=O)c1cc[nH]c1C
null
null
O
Aromatic Heterocycle Formation
OtherReaction
2633cdec1426893628fe136129d1edcddc4b21c65927a590f43ab5196c42f086
f397f35add667cd2079cc0f5c10fd9068989f947555f4b5ec67f80071ec94898
c1cc[nH]c1
C-C(=O)-O-[CH;D2;+0:1]=[CH2;D1;+0:2].O=[C;H0;D3;+0:3](-[C;D1;H3:4])-[CH2;D2;+0:5]-[C:6](=[O;D1;H0:7])-[#8:8]-[C:9].[NH3;D0;+0:10]>>[C:9]-[#8:8]-[C:6](=[O;D1;H0:7])-[c;H0;D3;+0:5]1:[cH;D2;+0:2]:[cH;D2;+0:1]:[nH;D2;+0:10]:[c;H0;D3;+0:3]:1-[C;D1;H3:4]
35
[{"value": 35.0, "product": "CC=1NC=CC1C(=O)OCC", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
Vinyl acetate (13.4 g) was added dropwise over 2 hr to bromine (25 g) under ice-cooling with stirring. The reaction mixture was further stirred at the same temperature for 1 hr. Ethyl 3-oxobutanoate (18.5 g) was added, and 25% aqueous ammonia solution (44 mL) was added dropwise over 1 hr. The reaction mixture was furth...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ester.Ester.Vinyl
Ester
null
c1cc[nH]c1
c1cc[nH]c1
HO-
O
null
null
C=COC(C)=O.CCOC(=O)CC(C)=O.N>O>CCOC(=O)c1cc[nH]c1C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2a6eeb3c376c4a268630653acdd2cd34
COC(=O)c1cc[nH]c1.O=C1CCC(=O)N1Br>>COC(=O)c1c[nH]c(Br)c1
N1C=C(C=C1)C(=O)OC.BrN1C(CCC1=O)=O.O>>BrC1=CC(=CN1)C(=O)OC
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][nH:7][cH:8][cH:10]1.O=C1CCC(=O)N1[Br:9]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][nH:7][c:8]([Br:9])[cH:10]1
COC(=O)c1cc[nH]c1.O=C1CCC(=O)N1Br
COC(=O)c1c[nH]c(Br)c1
null
N1=CC=CC=C1
O1CCCC1
Functional Group Interconversion
Bromination
40ba41cd9c6955f8bb4a47b285f327e8347ac41f3539d665e8b27d9300f356ae
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
c1cc[nH]c1
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#8:2]-[C:3](=[O;D1;H0:4])-[c:5]1:[c:6]:[cH;D2;+0:7]:[#7;a:8]:[c:9]:1>>[#8:2]-[C:3](=[O;D1;H0:4])-[c:5]1:[c:6]:[c;H0;D3;+0:7](-[Br;H0;D1;+0:1]):[#7;a:8]:[c:9]:1
62
[{"value": 62.0, "product": "BrC1=CC(=CN1)C(=O)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 61.7, "product": "BrC1=CC(=CN1)C(=O)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
A solution (30 mL) of methyl 1H-pyrrole-3-carboxylate (3.06 g) in tetrahydrofuran was cooled to −78° C., N-bromosuccinimide (4.38 g) and then pyridine (3 drops) were added, and the mixture was stirred at the same temperature for 1 hr. Water was added to the reaction mixture, and the mixture was extracted with ethyl ace...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1cc[nH]c1.C1CCNC1
c1cc[nH]c1
c1cc[nH]c1
HO-
N1=CC=CC=C1.O1CCCC1
null
1
COC(=O)c1cc[nH]c1.O=C1CCC(=O)N1Br>N1=CC=CC=C1.O1CCCC1>COC(=O)c1c[nH]c(Br)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-904e584988244852b2ce443b7b421560
COC(=O)c1c[nH]cc1C.O=C1CCC(=O)N1Br>>COC(=O)c1c[nH]c(Br)c1C
CC=1C(=CNC1)C(=O)OC.BrN1C(CCC1=O)=O>>BrC1=C(C(=CN1)C(=O)OC)C
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][nH:7][cH:8][c:10]1[CH3:11].O=C1CCC(=O)N1[Br:9]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][nH:7][c:8]([Br:9])[c:10]1[CH3:11]
COC(=O)c1c[nH]cc1C.O=C1CCC(=O)N1Br
COC(=O)c1c[nH]c(Br)c1C
null
null
null
Functional Group Interconversion
Bromination
40ba41cd9c6955f8bb4a47b285f327e8347ac41f3539d665e8b27d9300f356ae
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
c1cc[nH]c1
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#8:2]-[C:3](=[O;D1;H0:4])-[c:5]1:[c:6]:[#7;a:7]:[cH;D2;+0:8]:[c:9]:1-[C;D1;H3:10]>>[#8:2]-[C:3](=[O;D1;H0:4])-[c:5]1:[c:6]:[#7;a:7]:[c;H0;D3;+0:8](-[Br;H0;D1;+0:1]):[c:9]:1-[C;D1;H3:10]
31
[{"value": 31.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a similar operation as in Reference Example 22 and using methyl 4-methyl-1H-pyrrole-3-carboxylate (1.0 g) and N-bromosuccinimide (1.28 g), the title compound was obtained as a pale-yellow solid (yield 489 mg, 31%). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1cc[nH]c1.C1CCNC1
c1cc[nH]c1
c1cc[nH]c1
HO-
null
null
null
COC(=O)c1c[nH]cc1C.O=C1CCC(=O)N1Br>>COC(=O)c1c[nH]c(Br)c1C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7f6a8a451cf94b50be7fa1ea2b7f6126
CCOC(=O)c1cc[nH]c1C.O=C1CCC(=O)N1Br>>CCOC(=O)c1cc(Br)[nH]c1C
O.C(C)OCC.CC=1NC=CC1C(=O)OCC.BrN1C(CCC1=O)=O>>BrC1=CC(=C(N1)C)C(=O)OCC
[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][nH:10][c:11]1[CH3:12].O=C1CCC(=O)N1[Br:9]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][c:8]([Br:9])[nH:10][c:11]1[CH3:12]
CCOC(=O)c1cc[nH]c1C.O=C1CCC(=O)N1Br
CCOC(=O)c1cc(Br)[nH]c1C
null
null
O1CCCC1
Functional Group Interconversion
Bromination
40ba41cd9c6955f8bb4a47b285f327e8347ac41f3539d665e8b27d9300f356ae
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
c1cc[nH]c1
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#8:2]-[C:3](=[O;D1;H0:4])-[c:5]1:[c:6]:[#7;a:7]:[cH;D2;+0:8]:[c:9]:1>>[#8:2]-[C:3](=[O;D1;H0:4])-[c:5]1:[c:6]:[#7;a:7]:[c;H0;D3;+0:8](-[Br;H0;D1;+0:1]):[c:9]:1
97.5
[{"value": 97.0, "product": "BrC1=CC(=C(N1)C)C(=O)OCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 97.5, "product": "BrC1=CC(=C(N1)C)C(=O)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
To a solution of ethyl 2-methyl-1H-pyrrole-3-carboxylate (1.53 g) in tetrahydrofuran (20 mL) was added N-bromosuccinimide (1.78 g) at −78° C., and the mixture was stirred at the same temperature for 30 min. Water and diethyl ether were added to extract the reaction mixture. The extract was washed with saturated brine, ...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1cc[nH]c1.C1CCNC1
c1cc[nH]c1
c1cc[nH]c1
HO-
O1CCCC1
null
0.5
CCOC(=O)c1cc[nH]c1C.O=C1CCC(=O)N1Br>O1CCCC1>CCOC(=O)c1cc(Br)[nH]c1C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4e377dbb240c4fa980e16805795d7559
O=P(Cl)(Cl)Cl.O=S(=O)(O)c1cccnc1>>O=S(=O)(Cl)c1cccnc1
Cl.N1=CC(=CC=C1)S(=O)(=O)O.P(Cl)(Cl)(Cl)(Cl)Cl.P(=O)(Cl)(Cl)Cl>>Cl.N1=CC(=CC=C1)S(=O)(=O)Cl
O=P(Cl)(Cl)[Cl:5].O[S:3](=[O:2])(=[O:4])[c:6]1[cH:7][cH:8][cH:9][n:10][cH:11]1>>[O:2]=[S:3](=[O:4])([Cl:5])[c:6]1[cH:7][cH:8][cH:9][n:10][cH:11]1
O=P(Cl)(Cl)Cl.O=S(=O)(O)c1cccnc1
O=S(=O)(Cl)c1cccnc1
null
null
C(Cl)(Cl)Cl
Functional Group Interconversion
OtherReaction
1d60417dbcce8291d459a7fb34824cf29ea6f69a30ac46aeb585ac8e7b69013e
4a93b4a9749514113cd3dffa44b64f21b1f88d26b8739299bcad711fe7a13a1b
c1ccncc1
Cl-P(-Cl)(=O)-[Cl;H0;D1;+0:1].O-[S;H0;D4;+0:2](=[O;D1;H0:3])(=[O;D1;H0:4])-[c:5](:[c:6]):[c:7]:[#7;a:8]:[c:9]>>[Cl;H0;D1;+0:1]-[S;H0;D4;+0:2](=[O;D1;H0:3])(=[O;D1;H0:4])-[c:5](:[c:6]):[c:7]:[#7;a:8]:[c:9]
81
[{"value": 81.0, "product": "Cl.N1=CC(=CC=C1)S(=O)(=O)Cl", "details": "PERCENTYIELD", "is_desired": false}]
120
CELSIUS
8
HOUR
A mixture of 3-pyridinesulfonic acid (50.0 g), phosphorus pentachloride (80.0 g) and phosphorus oxychloride (100 mL) was stirred at 120° C. for 8 hr. Under a nitrogen atmosphere, the mixture was cooled to room temperature, and chloroform (dehydrated, 330 mL) was added. Hydrogen chloride was blown in, and the precipitat...
10.6084/m9.figshare.5104873.v1
null
Sulfonic acid
Sulfonyl halide
null
null
c1ccncc1
HCl
C(Cl)(Cl)Cl
120
8
O=P(Cl)(Cl)Cl.O=S(=O)(O)c1cccnc1>C(Cl)(Cl)Cl>O=S(=O)(Cl)c1cccnc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-685b563a3f044c4c814e1a24381beab1
COc1ccc(N)cn1.Cl.O=S=O>>COc1ccc(S(=O)(=O)Cl)cn1
S(=O)=O.NC=1C=CC(=NC1)OC.Cl.N(=O)[O-].[Na+]>>COC1=CC=C(C=N1)S(=O)(=O)Cl
N[c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[n:12][cH:11]1.[ClH:10].[S:7](=[O:8])=[O:9]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([S:7](=[O:8])(=[O:9])[Cl:10])[cH:11][n:12]1
COc1ccc(N)cn1.Cl.O=S=O
COc1ccc(S(=O)(=O)Cl)cn1
null
null
C(C)(=O)O
Heteroatom Alkylation and Arylation
OtherReaction
d44a4364e5511e440a48fb914cbd59017338faff430f0e7127e14fae8b0eff0a
49dcc8f7b4471977f8fe724b4dd774612c303d853f75a373d5b25cc7ccd4c205
c1ccncc1
N-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]:[c:6]:1.[ClH;D0;+0:7].[O;D1;H0:8]=[S;H0;D2;+0:9]=[O;D1;H0:10]>>[Cl;H0;D1;+0:7]-[S;H0;D4;+0:9](=[O;D1;H0:8])(=[O;D1;H0:10])-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]:[c:6]:1
51
[{"value": 51.0, "product": "COC1=CC=C(C=N1)S(=O)(=O)Cl", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
5-Amino-2-methoxypyridine (1.24 g) was dissolved in acetic acid (8.3 mL), and the mixture was stirred under ice-cooling. Concentrated hydrochloric acid (8.3 mL) was added, and an aqueous solution (5 mL) of sodium nitrite (689 mg) was added dropwise over 15 min while keeping the inside temperature at not higher than 10°...
10.6084/m9.figshare.5104873.v1
null
Primary amine
Sulfonyl halide
c1ccncc1
c1ccncc1
c1ccncc1
Other
C(C)(=O)O
null
null
COc1ccc(N)cn1.Cl.O=S=O>C(C)(=O)O>COc1ccc(S(=O)(=O)Cl)cn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-156979b5ed7b42a69b0af40d5cec0cb0
Cl.Nc1ccc(Cl)nc1.O=S=O>>O=S(=O)(Cl)c1ccc(Cl)nc1
N(=O)[O-].[Na+].NC=1C=CC(=NC1)Cl.Cl.S(=O)=O>>ClC1=CC=C(C=N1)S(=O)(=O)Cl
[ClH:4].N[c:5]1[cH:6][cH:7][c:8]([Cl:9])[n:10][cH:11]1.[O:1]=[S:2]=[O:3]>>[O:1]=[S:2](=[O:3])([Cl:4])[c:5]1[cH:6][cH:7][c:8]([Cl:9])[n:10][cH:11]1
Cl.Nc1ccc(Cl)nc1.O=S=O
O=S(=O)(Cl)c1ccc(Cl)nc1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
d44a4364e5511e440a48fb914cbd59017338faff430f0e7127e14fae8b0eff0a
49dcc8f7b4471977f8fe724b4dd774612c303d853f75a373d5b25cc7ccd4c205
c1ccncc1
N-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]:[c:6]:1.[ClH;D0;+0:7].[O;D1;H0:8]=[S;H0;D2;+0:9]=[O;D1;H0:10]>>[Cl;H0;D1;+0:7]-[S;H0;D4;+0:9](=[O;D1;H0:8])(=[O;D1;H0:10])-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]:[c:6]:1
58
[{"value": 58.0, "product": "ClC1=CC=C(C=N1)S(=O)(=O)Cl", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
Under ice-cooling, thionyl chloride (12 mL) was added dropwise over 1 hr to water (70 mL) and the mixture was stirred at room temperature for 12 hr to give a sulfur dioxide-containing solution. Separately, under ice-cooling, 5-amino-2-chloropyridine (5.0 g) was added to concentrated hydrochloric acid (40 mL) and the mi...
10.6084/m9.figshare.5104873.v1
null
Primary amine
Sulfonyl halide
c1ccncc1
c1ccncc1
c1ccncc1
Other
null
null
null
Cl.Nc1ccc(Cl)nc1.O=S=O>>O=S(=O)(Cl)c1ccc(Cl)nc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-35d51a9a1d2749fc9c60ce097cc97ef4
Cl.Nc1cccnc1Cl.O=S=O>>O=S(=O)(Cl)c1cccnc1Cl
N(=O)[O-].[Na+].NC=1C(=NC=CC1)Cl.Cl.S(=O)=O>>ClC1=NC=CC=C1S(=O)(=O)Cl
[ClH:4].N[c:5]1[cH:6][cH:7][cH:8][n:9][c:10]1[Cl:11].[O:1]=[S:2]=[O:3]>>[O:1]=[S:2](=[O:3])([Cl:4])[c:5]1[cH:6][cH:7][cH:8][n:9][c:10]1[Cl:11]
Cl.Nc1cccnc1Cl.O=S=O
O=S(=O)(Cl)c1cccnc1Cl
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
d44a4364e5511e440a48fb914cbd59017338faff430f0e7127e14fae8b0eff0a
49dcc8f7b4471977f8fe724b4dd774612c303d853f75a373d5b25cc7ccd4c205
c1ccncc1
N-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[#7;a:5]:[c:6]:1-[Cl;D1;H0:7].[ClH;D0;+0:8].[O;D1;H0:9]=[S;H0;D2;+0:10]=[O;D1;H0:11]>>[Cl;D1;H0:7]-[c:6]1:[#7;a:5]:[c:4]:[c:3]:[c:2]:[c;H0;D3;+0:1]:1-[S;H0;D4;+0:10](-[Cl;H0;D1;+0:8])(=[O;D1;H0:9])=[O;D1;H0:11]
42
[{"value": 42.0, "product": "ClC1=NC=CC=C1S(=O)(=O)Cl", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
Under ice-cooling, thionyl chloride (24 mL) was added dropwise over 1 hr to water (140 mL) and the mixture was stirred at room temperature for 12 hr to give a sulfur dioxide-containing solution. Separately, under ice-cooling, 3-amino-2-chloropyridine (10 g) was added to concentrated hydrochloric acid (80 mL) and the mi...
10.6084/m9.figshare.5104873.v1
null
Primary amine
Sulfonyl halide
c1ccncc1
c1ccncc1
c1ccncc1
Other
null
null
null
Cl.Nc1cccnc1Cl.O=S=O>>O=S(=O)(Cl)c1cccnc1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-870c5c31dd374e4eb91f07bbaff0a4e0
Cc1cc([N+](=O)[O-])cnc1Cl>>Cc1cc(N)cnc1Cl
[Cl-].[NH4+].ClC1=NC=C(C=C1C)[N+](=O)[O-]>>ClC1=C(C=C(C=N1)N)C
O=[N+:5]([O-])[c:4]1[cH:3][c:2]([CH3:1])[c:8]([Cl:9])[n:7][cH:6]1>>[CH3:1][c:2]1[cH:3][c:4]([NH2:5])[cH:6][n:7][c:8]1[Cl:9]
Cc1cc([N+](=O)[O-])cnc1Cl
Cc1cc(N)cnc1Cl
null
null
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccncc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]:[#7;a:5]:[c:6]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]:[#7;a:5]:[c:6]
42
[{"value": 42.0, "product": "ClC1=C(C=C(C=N1)N)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 41.5, "product": "ClC1=C(C=C(C=N1)N)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
5
MINUTE
Reduced iron (793 mg) was added to an aqueous solution (25 mL) of ammonium chloride (1.27 g), and the mixture was stirred at room temperature for 5 min. A solution (10 mL) of 2-chloro-3-methyl-5-nitropyridine (816 mg) in methanol was added dropwise over 10 min. The reaction mixture was stirred at 40° C. for 20 min and ...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccncc1
Other
CO
null
0.083333
Cc1cc([N+](=O)[O-])cnc1Cl>CO>Cc1cc(N)cnc1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c7ea0e95dd0b44798fc29a0b9c8d4253
Cc1cc(N)cnc1Cl.Cl.O=S=O>>Cc1cc(S(=O)(=O)Cl)cnc1Cl
S(=O)=O.ClC1=C(C=C(C=N1)N)C.Cl.N(=O)[O-].[Na+]>>ClC1=C(C=C(C=N1)S(=O)(=O)Cl)C
N[c:4]1[cH:3][c:2]([CH3:1])[c:11]([Cl:12])[n:10][cH:9]1.[ClH:8].[S:5](=[O:6])=[O:7]>>[CH3:1][c:2]1[cH:3][c:4]([S:5](=[O:6])(=[O:7])[Cl:8])[cH:9][n:10][c:11]1[Cl:12]
Cc1cc(N)cnc1Cl.Cl.O=S=O
Cc1cc(S(=O)(=O)Cl)cnc1Cl
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
d44a4364e5511e440a48fb914cbd59017338faff430f0e7127e14fae8b0eff0a
49dcc8f7b4471977f8fe724b4dd774612c303d853f75a373d5b25cc7ccd4c205
c1ccncc1
N-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[#7;a:5]:[c:6]:1.[ClH;D0;+0:7].[O;D1;H0:8]=[S;H0;D2;+0:9]=[O;D1;H0:10]>>[Cl;H0;D1;+0:7]-[S;H0;D4;+0:9](=[O;D1;H0:8])(=[O;D1;H0:10])-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[#7;a:5]:[c:6]:1
62
[{"value": 62.0, "product": "ClC1=C(C=C(C=N1)S(=O)(=O)Cl)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
Under ice-cooling, thionyl chloride (0.6 mL) was added dropwise over 30 min to water (3.4 mL). The mixture was stirred at room temperature for 12 hr to give a sulfur dioxide-containing solution. Separately, under ice-cooling, 6-chloro-5-methylpyridine-3-amine (278 mg) was added to concentrated hydrochloric acid (6 mL) ...
10.6084/m9.figshare.5104873.v1
null
Primary amine
Sulfonyl halide
c1ccncc1
c1ccncc1
c1ccncc1
Other
null
null
null
Cc1cc(N)cnc1Cl.Cl.O=S=O>>Cc1cc(S(=O)(=O)Cl)cnc1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ef15361f7a62441d899e6da0afee91eb
O=S(=O)(O)O.Sc1ccccn1.[O-]Cl>>O=S(=O)(Cl)c1ccccn1
SC1=NC=CC=C1.S(O)(O)(=O)=O.Cl[O-].[Na+]>>N1=C(C=CC=C1)S(=O)(=O)Cl
O=S(O)(O)=[O:3].[SH:2][c:5]1[cH:6][cH:7][cH:8][cH:9][n:10]1.[O-:1][Cl:4]>>[O:1]=[S:2](=[O:3])([Cl:4])[c:5]1[cH:6][cH:7][cH:8][cH:9][n:10]1
O=S(=O)(O)O.Sc1ccccn1.[O-]Cl
O=S(=O)(Cl)c1ccccn1
null
null
O
Oxidation
OtherReaction
9785de8c4af497b47fef775da94901f552247c79b12446361bd1c0f569fb21a2
00ceeb3b5a6ffef49234435732248538ad1b48dd29750ec1526974fa138e885a
c1ccncc1
O-S(-O)(=O)=[O;H0;D1;+0:1].[Cl;H0;D1;+0:2]-[O-;H0;D1:3].[SH;D1;+0:4]-[c:5](:[c:6]):[#7;a:7]:[c:8]>>[Cl;H0;D1;+0:2]-[S;H0;D4;+0:4](=[O;H0;D1;+0:3])(=[O;H0;D1;+0:1])-[c:5](:[c:6]):[#7;a:7]:[c:8]
77
[{"value": 77.0, "product": "N1=C(C=CC=C1)S(=O)(=O)Cl", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
Under ice-cooling, 2-mercaptopyridine (2.0 g) was added to sulfuric acid (50 mL) and the mixture was stirred. Sodium hypochlorite solution (chlorine content 5%, 126 mL) was added dropwise over 1.5 hr, and the mixture was further stirred at the same temperature for 30 min. The reaction mixture was diluted with water (10...
10.6084/m9.figshare.5104873.v1
null
Aromatic thiol
Sulfonyl halide
null
null
c1ccncc1
HO-
O
null
null
O=S(=O)(O)O.Sc1ccccn1.[O-]Cl>O>O=S(=O)(Cl)c1ccccn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b0800cd075b74b94b7340e01104e400e
CCOC(=O)c1c[nH]c(-c2ccccc2)c1.O=S(=O)(F)c1ccc(Cl)nn1>>CCOC(=O)c1cc(-c2ccccc2)n(S(=O)(=O)c2cccnn2)c1
ClC1=CC=C(N=N1)S(=O)(=O)F.C(O)([O-])=O.[Na+].C1COCCOCCOCCOCCO1.[H-].[Na+].NN.C1(=CC=CC=C1)C1=CC(=CN1)C(=O)OCC>>C1(=CC=CC=C1)C1=CC(=CN1S(=O)(=O)C=1N=NC=CC1)C(=O)OCC
[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][c:8](-[c:9]2[cH:10][cH:11][cH:12][cH:13][cH:14]2)[nH:15][cH:25]1.F[S:16](=[O:17])(=[O:18])[c:19]1[cH:20][cH:21][c:22](Cl)[n:23][n:24]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][c:8](-[c:9]2[cH:10][cH:11][cH:12][cH:13][cH:14]2)[n:15]([S:16](=[O:17])(=[O:18])[c:19]2[cH:20]...
CCOC(=O)c1c[nH]c(-c2ccccc2)c1.O=S(=O)(F)c1ccc(Cl)nn1
CCOC(=O)c1cc(-c2ccccc2)n(S(=O)(=O)c2cccnn2)c1
null
null
O1CCCC1
Acylation
OtherReaction
a029c3e19ecd4bb7a8b7eda76bd36682476a6f6535504b6e2764312ea6c234fc
3d2c04f63ac9e2f3df734bfe73fabc984c30969d75ff1d2ce6780c93e45e2f3f
O=S(=O)(c1cccnn1)n1cccc1-c1ccccc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[#7;a:3]:[c:4](-[S;H0;D4;+0:5](-F)(=[O;D1;H0:6])=[O;D1;H0:7]):[c:8]:[c:9]:1.[#8:10]-[C:11](=[O;D1;H0:12])-[c:13]1:[c:14]:[nH;D2;+0:15]:[c:16](-[c:17]):[c:18]:1>>[#8:10]-[C:11](=[O;D1;H0:12])-[c:13]1:[c:14]:[n;H0;D3;+0:15](-[S;H0;D4;+0:5](=[O;D1;H0:6])(=[O;D1;H0:7])-[c:4]2:[#7;a:3]:[#7;a:2]:[...
34.8
[{"value": 24.0, "product": "C1(=CC=CC=C1)C1=CC(=CN1S(=O)(=O)C=1N=NC=CC1)C(=O)OCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 34.8, "product": "C1(=CC=CC=C1)C1=CC(=CN1S(=O)(=O)C=1N=NC=CC1)C(=O)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
Ethyl 5-phenyl-1H-pyrrole-3-carboxylate (1.06 g) was dissolved in tetrahydrofuran (30 mL), sodium hydride (60% in oil, 300 mg) was added and the mixture was stirred at room temperature for 15 min. 15-Crown-5 (1.52 mL) was added and the mixture was further stirred at the same temperature for 15 min. 6-Chloropyridazine-3...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Sulfonyl halide
null
c1cc[nH]c1.c1ccnnc1
c1cc[nH]c1.c1ccnnc1
c1cc[nH]c1.c1ccccc1.c1ccnnc1
Other
O1CCCC1
null
0.25
CCOC(=O)c1c[nH]c(-c2ccccc2)c1.O=S(=O)(F)c1ccc(Cl)nn1>O1CCCC1>CCOC(=O)c1cc(-c2ccccc2)n(S(=O)(=O)c2cccnn2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a0cd5a3f20ee49d6aab74a710f332afe
CCOC(=O)c1cc[nH]c1C.O=S(=O)(Cl)c1ccccc1>>CCOC(=O)c1ccn(S(=O)(=O)c2ccccc2)c1C
C1(=CC=CC=C1)S(=O)(=O)Cl.CC=1NC=CC1C(=O)OCC.[H-].[Na+]>>CC=1N(C=CC1C(=O)OCC)S(=O)(=O)C1=CC=CC=C1
[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][nH:9][c:19]1[CH3:20].Cl[S:10](=[O:11])(=[O:12])[c:13]1[cH:14][cH:15][cH:16][cH:17][cH:18]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][n:9]([S:10](=[O:11])(=[O:12])[c:13]2[cH:14][cH:15][cH:16][cH:17][cH:18]2)[c:19]1[CH3:20]
CCOC(=O)c1cc[nH]c1C.O=S(=O)(Cl)c1ccccc1
CCOC(=O)c1ccn(S(=O)(=O)c2ccccc2)c1C
null
null
null
Acylation
OtherReaction
40c00ec44b7af41885dbd1ffd066e14223cf28d90060492536c6496a8e914910
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1ccccc1)n1cccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[#8:7]-[C:8](=[O;D1;H0:9])-[c:10]1:[c:11]:[c:12]:[nH;D2;+0:13]:[c:14]:1-[C;D1;H3:15]>>[#8:7]-[C:8](=[O;D1;H0:9])-[c:10]1:[c:11]:[c:12]:[n;H0;D3;+0:13](-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]):[c:14]:1-[C;D1;H3:15]
85
[{"value": 85.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a similar operation as in Reference Example 41 and using ethyl 2-methyl-1H-pyrrole-3-carboxylate (8.81 g), sodium hydride (60% in oil, 2.58 g) and benzenesulfonyl chloride (7.8 mL), the title compound was obtained as white crystals (yield 14.3 g, 85%). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1c[nH]cc1
c1c[nH]cc1.c1ccccc1
HCl
null
null
null
CCOC(=O)c1cc[nH]c1C.O=S(=O)(Cl)c1ccccc1>>CCOC(=O)c1ccn(S(=O)(=O)c2ccccc2)c1C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-51b0a26a2bbc4d6f88a66fbda2f9cd5c
CCOC(=O)c1cc(Br)[nH]c1C.O=S(=O)(Cl)c1cccnc1>>CCOC(=O)c1cc(Br)n(S(=O)(=O)c2cccnc2)c1C
Cl.N1=CC(=CC=C1)S(=O)(=O)Cl.BrC1=CC(=C(N1)C)C(=O)OCC.[H-].[Na+].C(O)([O-])=O.[Na+].C1COCCOCCOCCOCCO1>>BrC1=CC(=C(N1S(=O)(=O)C=1C=NC=CC1)C)C(=O)OCC
[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][c:8]([Br:9])[nH:10][c:20]1[CH3:21].Cl[S:11](=[O:12])(=[O:13])[c:14]1[cH:15][cH:16][cH:17][n:18][cH:19]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][c:8]([Br:9])[n:10]([S:11](=[O:12])(=[O:13])[c:14]2[cH:15][cH:16][cH:17][n:18][cH:19]2)[c:20]1[CH3:21]
CCOC(=O)c1cc(Br)[nH]c1C.O=S(=O)(Cl)c1cccnc1
CCOC(=O)c1cc(Br)n(S(=O)(=O)c2cccnc2)c1C
null
null
O1CCCC1
Acylation
OtherReaction
40c00ec44b7af41885dbd1ffd066e14223cf28d90060492536c6496a8e914910
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cccnc1)n1cccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8].[#8:9]-[C:10](=[O;D1;H0:11])-[c:12]1:[c:13]:[c:14](-[Br;D1;H0:15]):[nH;D2;+0:16]:[c:17]:1-[C;D1;H3:18]>>[#8:9]-[C:10](=[O;D1;H0:11])-[c:12]1:[c:13]:[c:14](-[Br;D1;H0:15]):[n;H0;D3;+0:16](-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[...
64
[{"value": 64.0, "product": "BrC1=CC(=C(N1S(=O)(=O)C=1C=NC=CC1)C)C(=O)OCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 63.6, "product": "BrC1=CC(=C(N1S(=O)(=O)C=1C=NC=CC1)C)C(=O)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
Ethyl 5-bromo-2-methyl-1H-pyrrole-3-carboxylate (2.26 g) was dissolved in tetrahydrofuran (100 mL), sodium hydride (60% in oil, 1.16 g) was added and the mixture was stirred at room temperature for 15 min. 15-Crown-5 (5.90 mL) was added and the mixture was further stirred at the same temperature for 15 min. 3-Pyridines...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1c[nH]cc1
c1c[nH]cc1.c1ccncc1
HCl
O1CCCC1
null
0.25
CCOC(=O)c1cc(Br)[nH]c1C.O=S(=O)(Cl)c1cccnc1>O1CCCC1>CCOC(=O)c1cc(Br)n(S(=O)(=O)c2cccnc2)c1C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5b113a56f9294f2abf9dabf6e5fcda88
CCOC(=O)c1cc(Br)n(S(=O)(=O)c2cccnc2)c1C.OB(O)c1ccccc1>>CCOC(=O)c1cc(-c2ccccc2)n(S(=O)(=O)c2cccnc2)c1C
BrC1=CC(=C(N1S(=O)(=O)C=1C=NC=CC1)C)C(=O)OCC.C1(=CC=CC=C1)B(O)O.C([O-])([O-])=O.[Na+].[Na+].O>>CC=1N(C(=CC1C(=O)OCC)C1=CC=CC=C1)S(=O)(=O)C=1C=NC=CC1
Br[c:8]1[cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[c:25]([CH3:26])[n:15]1[S:16](=[O:17])(=[O:18])[c:19]1[cH:20][cH:21][cH:22][n:23][cH:24]1.OB(O)[c:9]1[cH:10][cH:11][cH:12][cH:13][cH:14]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][c:8](-[c:9]2[cH:10][cH:11][cH:12][cH:13][cH:14]2)[n:15]([S:16](=[O:17])(=[O:18])[c:...
CCOC(=O)c1cc(Br)n(S(=O)(=O)c2cccnc2)c1C.OB(O)c1ccccc1
CCOC(=O)c1cc(-c2ccccc2)n(S(=O)(=O)c2cccnc2)c1C
null
null
COCCOC
C-C Coupling
Suzuki coupling with boronic acids
b2d7c68422e63d91324e9f95cf31db744bedd9bd92be56bb43ec6d6dd2e086c2
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[C:4](-[#8:5])=[O;D1;H0:6]):[c:7]:[#7;a:8]:1-[#16:9].O-B(-O)-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]>>[#16:9]-[#7;a:8]1:[c:7]:[c:3](-[C:4](-[#8:5])=[O;D1;H0:6]):[c:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]
106.6
[{"value": 100.0, "product": "CC=1N(C(=CC1C(=O)OCC)C1=CC=CC=C1)S(=O)(=O)C=1C=NC=CC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 106.6, "product": "CC=1N(C(=CC1C(=O)OCC)C1=CC=CC=C1)S(=O)(=O)C=1C=NC=CC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
40
MINUTE
A suspension of ethyl 5-bromo-2-methyl-1-(pyridin-3-ylsulfonyl)-1H-pyrrole-3-carboxylate (2.26 g), phenylboronic acid (1.54 g), dichloro[bis(triphenylphosphine)]palladium (211 mg) and sodium carbonate (1.91 g) in 1,2-dimethoxyethane (20 mL)-water (10 mL) was stirred at 80° C. for 40 min. After cooling, the reaction mix...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1c[nH]cc1.c1ccccc1
c1c[nH]cc1.c1ccccc1
c1c[nH]cc1.c1ccccc1.c1ccncc1
HBr.B
COCCOC
80
0.666667
CCOC(=O)c1cc(Br)n(S(=O)(=O)c2cccnc2)c1C.OB(O)c1ccccc1>COCCOC>CCOC(=O)c1cc(-c2ccccc2)n(S(=O)(=O)c2cccnc2)c1C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7ce408ff2a7a4fad8ca77311f2254f40
COC(=O)c1cc(Br)n(S(=O)(=O)c2ccccc2)c1>>O=S(=O)(c1ccccc1)n1cc(CO)cc1Br
Cl.[H-].C(C(C)C)[Al+]CC(C)C.BrC1=CC(=CN1S(=O)(=O)C1=CC=CC=C1)C(=O)OC>>BrC1=CC(=CN1S(=O)(=O)C1=CC=CC=C1)CO
CO[C:13]([c:12]1[cH:11][n:10]([S:2](=[O:1])(=[O:3])[c:4]2[cH:5][cH:6][cH:7][cH:8][cH:9]2)[c:16]([Br:17])[cH:15]1)=[O:14]>>[O:1]=[S:2](=[O:3])([c:4]1[cH:5][cH:6][cH:7][cH:8][cH:9]1)[n:10]1[cH:11][c:12]([CH2:13][OH:14])[cH:15][c:16]1[Br:17]
COC(=O)c1cc(Br)n(S(=O)(=O)c2ccccc2)c1
O=S(=O)(c1ccccc1)n1cc(CO)cc1Br
null
null
O1CCCC1.C1(=CC=CC=C1)C
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
O=S(=O)(c1ccccc1)n1cccc1
C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3]1:[c:4]:[#7;a:5](-[#16:6]):[c:7]:[c:8]:1>>[#16:6]-[#7;a:5]1:[c:4]:[c:3](-[CH2;D2;+0:1]-[OH;D1;+0:2]):[c:8]:[c:7]:1
108.9
[{"value": 100.0, "product": "BrC1=CC(=CN1S(=O)(=O)C1=CC=CC=C1)CO", "details": "PERCENTYIELD", "is_desired": false}, {"value": 108.9, "product": "BrC1=CC(=CN1S(=O)(=O)C1=CC=CC=C1)CO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-78
CELSIUS
1
HOUR
A solution (80 mL) of methyl 5-bromo-1-(phenylsulfonyl)-1H-pyrrole-3-carboxylate (7.1 g) in tetrahydrofuran was cooled to −78° C., a 1.5 mol/L solution (42 mL) of diisobutylaluminum hydride in toluene was added dropwise over 30 min and the mixture was further stirred at −78° C. for 1 hr. 1 mol/L hydrochloric acid (20 m...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
c1ccccc1.c1cc[nH]c1
Other
O1CCCC1.C1(=CC=CC=C1)C
-78
1
COC(=O)c1cc(Br)n(S(=O)(=O)c2ccccc2)c1>O1CCCC1.C1(=CC=CC=C1)C>O=S(=O)(c1ccccc1)n1cc(CO)cc1Br
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1d33ad461f684e69859d49638e5ac872
CCOC(=O)c1ccn(S(=O)(=O)c2ccccc2)c1C>>Cc1c(CO)ccn1S(=O)(=O)c1ccccc1
CC=1N(C=CC1C(=O)OCC)S(=O)(=O)C1=CC=CC=C1.C1(=CC=CC=C1)C.[H-].C(C(C)C)[Al+]CC(C)C>>CC=1N(C=CC1CO)S(=O)(=O)C1=CC=CC=C1
CCO[C:4]([c:3]1[c:2]([CH3:1])[n:8]([S:9](=[O:10])(=[O:11])[c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[cH:7][cH:6]1)=[O:5]>>[CH3:1][c:2]1[c:3]([CH2:4][OH:5])[cH:6][cH:7][n:8]1[S:9](=[O:10])(=[O:11])[c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1
CCOC(=O)c1ccn(S(=O)(=O)c2ccccc2)c1C
Cc1c(CO)ccn1S(=O)(=O)c1ccccc1
null
null
null
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
O=S(=O)(c1ccccc1)n1cccc1
C-C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3]1:[c:4]:[c:5]:[#7;a:6](-[#16:7]):[c:8]:1-[C;D1;H3:9]>>[#16:7]-[#7;a:6]1:[c:5]:[c:4]:[c:3](-[CH2;D2;+0:1]-[OH;D1;+0:2]):[c:8]:1-[C;D1;H3:9]
96
[{"value": 96.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a similar operation as in Reference Example 13 and using ethyl 2-methyl-1-(phenylsulfonyl)-1H-pyrrole-3-carboxylate (8.05 g) and 1.5 mol/L diisobutylaluminum hydride toluene solution (55 mL), the title compound was obtained as white crystals (yield 6.61 g, 96%). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
c1c[nH]cc1.c1ccccc1
HO-
null
null
null
CCOC(=O)c1ccn(S(=O)(=O)c2ccccc2)c1C>>Cc1c(CO)ccn1S(=O)(=O)c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-35771c8ef4bf4af6a1e4fe3ca0060164
O=S(=O)(c1ccccc1)n1cc(CO)cc1Br>>O=Cc1cc(Br)n(S(=O)(=O)c2ccccc2)c1
BrC1=CC(=CN1S(=O)(=O)C1=CC=CC=C1)CO.O.C[N+]1(CCOCC1)[O-]>>BrC1=CC(=CN1S(=O)(=O)C1=CC=CC=C1)C=O
[OH:1][CH2:2][c:3]1[cH:4][c:5]([Br:6])[n:7]([S:8](=[O:9])(=[O:10])[c:11]2[cH:12][cH:13][cH:14][cH:15][cH:16]2)[cH:17]1>>[O:1]=[CH:2][c:3]1[cH:4][c:5]([Br:6])[n:7]([S:8](=[O:9])(=[O:10])[c:11]2[cH:12][cH:13][cH:14][cH:15][cH:16]2)[cH:17]1
O=S(=O)(c1ccccc1)n1cc(CO)cc1Br
O=Cc1cc(Br)n(S(=O)(=O)c2ccccc2)c1
null
[Ru](=O)(=O)(=O)[O-].C(CC)[N+](CCC)(CCC)CCC
C(C)#N
Oxidation
Oxidation or Dehydrogenation of Alcohols to Aldehydes and Ketones
41bfa9deea81b465c88ad21fdfb64a2e1ba29490558cf430df132cb98b4a538b
0a03c6724c1862e8f86d4a463afda55b8e067dc6cb42597b472eb7cabc03eda3
O=S(=O)(c1ccccc1)n1cccc1
[#16:1]-[#7;a:2]1:[c:3]:[c:4](-[CH2;D2;+0:5]-[OH;D1;+0:6]):[c:7]:[c:8]:1>>[#16:1]-[#7;a:2]1:[c:3]:[c:4](-[CH;D2;+0:5]=[O;H0;D1;+0:6]):[c:7]:[c:8]:1
71
[{"value": 71.0, "product": "BrC1=CC(=CN1S(=O)(=O)C1=CC=CC=C1)C=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 65.2, "product": "BrC1=CC(=CN1S(=O)(=O)C1=CC=CC=C1)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
To a solution (80 mL) of [5-bromo-1-(phenylsulfonyl)-1H-pyrrol-3-yl]methanol (7.1 g) in acetonitrile were added tetra-n-propylammonium perruthenate (0.63 g), N-methylmorpholine N-oxide hydrate (4.2 g) and molecular sieves 4A powder (3.5 g), and the mixture was stirred at room temperature for 2 hr. The reaction mixture ...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Aldehyde
null
null
c1cc[nH]c1.c1ccccc1
null
[Ru](=O)(=O)(=O)[O-].C(CC)[N+](CCC)(CCC)CCC.C(C)#N
null
2
O=S(=O)(c1ccccc1)n1cc(CO)cc1Br>[Ru](=O)(=O)(=O)[O-].C(CC)[N+](CCC)(CCC)CCC.C(C)#N>O=Cc1cc(Br)n(S(=O)(=O)c2ccccc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-cef4b78ee4f94aa9ab2bc95d72810267
Cc1c(C=O)cn(S(=O)(=O)c2ccccc2)c1Br.OB(O)c1ccccc1>>Cc1c(C=O)c[nH]c1-c1ccccc1
BrC1=C(C(=CN1S(=O)(=O)C1=CC=CC=C1)C=O)C.C1(=CC=CC=C1)B(O)O.C([O-])([O-])=O.[Na+].[Na+].[OH-].[Na+]>>CC=1C(=CNC1C1=CC=CC=C1)C=O
O=S(=O)(c1ccccc1)[n:7]1[cH:6][c:3]([CH:4]=[O:5])[c:2]([CH3:1])[c:8]1Br.OB(O)[c:9]1[cH:10][cH:11][cH:12][cH:13][cH:14]1>>[CH3:1][c:2]1[c:3]([CH:4]=[O:5])[cH:6][nH:7][c:8]1-[c:9]1[cH:10][cH:11][cH:12][cH:13][cH:14]1
Cc1c(C=O)cn(S(=O)(=O)c2ccccc2)c1Br.OB(O)c1ccccc1
Cc1c(C=O)c[nH]c1-c1ccccc1
null
null
O.COCCOC
C-C Coupling
OtherReaction
10cbc4045254db5758344435c8b38bca11a334689db1f09754719c83db557e43
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc[nH]2)cc1
Br-[c;H0;D3;+0:1]1:[c:2](-[C;D1;H3:3]):[c:4](-[C:5]=[O;D1;H0:6]):[c:7]:[n;H0;D3;+0:8]:1-S(=O)(=O)-c1:c:c:c:c:c:1.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]>>[C;D1;H3:3]-[c:2]1:[c:4](-[C:5]=[O;D1;H0:6]):[c:7]:[nH;D2;+0:8]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]
81.1
[{"value": 69.0, "product": "CC=1C(=CNC1C1=CC=CC=C1)C=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 81.1, "product": "CC=1C(=CNC1C1=CC=CC=C1)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
1
HOUR
A suspension of 5-bromo-4-methyl-1-(phenylsulfonyl)-1H-pyrrole-3-carbaldehyde (1.78 g), phenylboronic acid (1.37 g), dichloro[bis(triphenylphosphine)]palladium (0.19 g) and sodium carbonate (1.72 g) in 1,2-dimethoxyethane (30 mL)-water (10 mL) was stirred at 100° C. for 1 hr. 8 mol/L aqueous sodium hydroxide solution (...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1cc[nH]c1.c1ccccc1
c1cc[nH]c1.c1ccccc1
c1cc[nH]c1.c1ccccc1
HBr.B
O.COCCOC
100
1
Cc1c(C=O)cn(S(=O)(=O)c2ccccc2)c1Br.OB(O)c1ccccc1>O.COCCOC>Cc1c(C=O)c[nH]c1-c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-018c2b5f131e41e688d594a36866654a
Cc1c(CO)ccn1S(=O)(=O)c1ccccc1>>Cc1c(C=O)ccn1S(=O)(=O)c1ccccc1
CC=1N(C=CC1CO)S(=O)(=O)C1=CC=CC=C1.CS(=O)C.C(O)([O-])=O.[Na+]>>CC=1N(C=CC1C=O)S(=O)(=O)C1=CC=CC=C1
[CH3:1][c:2]1[c:3]([CH2:4][OH:5])[cH:6][cH:7][n:8]1[S:9](=[O:10])(=[O:11])[c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1>>[CH3:1][c:2]1[c:3]([CH:4]=[O:5])[cH:6][cH:7][n:8]1[S:9](=[O:10])(=[O:11])[c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1
Cc1c(CO)ccn1S(=O)(=O)c1ccccc1
Cc1c(C=O)ccn1S(=O)(=O)c1ccccc1
null
null
C(C)N(CC)CC
Oxidation
Oxidation or Dehydrogenation of Alcohols to Aldehydes and Ketones
41bfa9deea81b465c88ad21fdfb64a2e1ba29490558cf430df132cb98b4a538b
0a03c6724c1862e8f86d4a463afda55b8e067dc6cb42597b472eb7cabc03eda3
O=S(=O)(c1ccccc1)n1cccc1
[#16:1]-[#7;a:2]1:[c:3]:[c:4]:[c:5](-[CH2;D2;+0:6]-[OH;D1;+0:7]):[c:8]:1-[C;D1;H3:9]>>[#16:1]-[#7;a:2]1:[c:3]:[c:4]:[c:5](-[CH;D2;+0:6]=[O;H0;D1;+0:7]):[c:8]:1-[C;D1;H3:9]
84
[{"value": 84.0, "product": "CC=1N(C=CC1C=O)S(=O)(=O)C1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 83.7, "product": "CC=1N(C=CC1C=O)S(=O)(=O)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
12
HOUR
To a mixture of [2-methyl-1-(phenylsulfonyl)-1H-pyrrol-3-yl]methanol (6.35 g), dimethyl sulfoxide (50 mL) and triethylamine (25 mL) was added sulfur trioxide-pyridine complex (4.57 g), and the mixture was stirred at room temperature for 12 hr. Saturated aqueous sodium hydrogencarbonate solution was added to the reactio...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Aldehyde
null
null
c1c[nH]cc1.c1ccccc1
null
C(C)N(CC)CC
null
12
Cc1c(CO)ccn1S(=O)(=O)c1ccccc1>C(C)N(CC)CC>Cc1c(C=O)ccn1S(=O)(=O)c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0c951f45b1dc459f9763ed1bcc0b6ad9
Cc1[nH]ccc1C=O.O=S(=O)(Cl)c1cccnc1>>Cc1c(C=O)ccn1S(=O)(=O)c1cccnc1
C1COCCOCCOCCOCCO1.CC=1NC=CC1C=O.Cl.N1=CC(=CC=C1)S(=O)(=O)Cl.[H-].[Na+]>>CC=1N(C=CC1C=O)S(=O)(=O)C=1C=NC=CC1
[CH3:1][c:2]1[c:3]([CH:4]=[O:5])[cH:6][cH:7][nH:8]1.Cl[S:9](=[O:10])(=[O:11])[c:12]1[cH:13][cH:14][cH:15][n:16][cH:17]1>>[CH3:1][c:2]1[c:3]([CH:4]=[O:5])[cH:6][cH:7][n:8]1[S:9](=[O:10])(=[O:11])[c:12]1[cH:13][cH:14][cH:15][n:16][cH:17]1
Cc1[nH]ccc1C=O.O=S(=O)(Cl)c1cccnc1
Cc1c(C=O)ccn1S(=O)(=O)c1cccnc1
null
null
null
Acylation
OtherReaction
40c00ec44b7af41885dbd1ffd066e14223cf28d90060492536c6496a8e914910
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cccnc1)n1cccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8].[C;D1;H3:9]-[c:10]1:[nH;D2;+0:11]:[c:12]:[c:13]:[c:14]:1-[C:15]=[O;D1;H0:16]>>[C;D1;H3:9]-[c:10]1:[c:14](-[C:15]=[O;D1;H0:16]):[c:13]:[c:12]:[n;H0;D3;+0:11]:1-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8]
44
[{"value": 44.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a similar reaction as in Reference Example 44 and using 2-methyl-1H-pyrrole-3-carbaldehyde (1.10 g), sodium hydride (60% in oil, 1.20 g), 15-crown-5 (6.0 mL) and pyridin-3-ylsulfonyl chloride hydrochloride (3.22 g), the title compound was obtained as white crystals (yield 1.10 g, 44%). Conditions: See reaction.notes...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1c[nH]cc1
c1c[nH]cc1.c1ccncc1
HCl
null
null
null
Cc1[nH]ccc1C=O.O=S(=O)(Cl)c1cccnc1>>Cc1c(C=O)ccn1S(=O)(=O)c1cccnc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-96d7ec4598274ba8b48a578f1317ae81
Cc1c(C=O)ccn1S(=O)(=O)c1cccnc1.O=C1CCC(=O)N1Br>>Cc1c(C=O)cc(Br)n1S(=O)(=O)c1cccnc1
O.CC=1N(C=CC1C=O)S(=O)(=O)C=1C=NC=CC1.BrN1C(CCC1=O)=O>>BrC1=CC(=C(N1S(=O)(=O)C=1C=NC=CC1)C)C=O
[CH3:1][c:2]1[c:3]([CH:4]=[O:5])[cH:6][cH:7][n:9]1[S:10](=[O:11])(=[O:12])[c:13]1[cH:14][cH:15][cH:16][n:17][cH:18]1.O=C1CCC(=O)N1[Br:8]>>[CH3:1][c:2]1[c:3]([CH:4]=[O:5])[cH:6][c:7]([Br:8])[n:9]1[S:10](=[O:11])(=[O:12])[c:13]1[cH:14][cH:15][cH:16][n:17][cH:18]1
Cc1c(C=O)ccn1S(=O)(=O)c1cccnc1.O=C1CCC(=O)N1Br
Cc1c(C=O)cc(Br)n1S(=O)(=O)c1cccnc1
null
null
CN(C=O)C
Functional Group Interconversion
Bromination
45b120e1defda7dfd188f9d58cce4a0f02402540683f8cdf07342faf62007b1f
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=S(=O)(c1cccnc1)n1cccc1
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#16:2]-[#7;a:3]1:[c:4]:[c:5](-[C:6]=[O;D1;H0:7]):[c:8]:[cH;D2;+0:9]:1>>[#16:2]-[#7;a:3]1:[c:4]:[c:5](-[C:6]=[O;D1;H0:7]):[c:8]:[c;H0;D3;+0:9]:1-[Br;H0;D1;+0:1]
53
[{"value": 53.0, "product": "BrC1=CC(=C(N1S(=O)(=O)C=1C=NC=CC1)C)C=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 52.7, "product": "BrC1=CC(=C(N1S(=O)(=O)C=1C=NC=CC1)C)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a solution of 2-methyl-1-(pyridin-3-ylsulfonyl)-1H-pyrrole-3-carbaldehyde (974 mg) in N,N-dimethylformamide (10 mL) was added N-bromosuccinimide (1.17 g) at 0° C., and the mixture was stirred at room temperature for 1 hr. Water was added to the reaction mixture, and the mixture was extracted with ethyl acetate. The ...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1c[nH]cc1.C1CCNC1
c1c[nH]cc1
c1c[nH]cc1.c1ccncc1
HO-
CN(C=O)C
null
1
Cc1c(C=O)ccn1S(=O)(=O)c1cccnc1.O=C1CCC(=O)N1Br>CN(C=O)C>Cc1c(C=O)cc(Br)n1S(=O)(=O)c1cccnc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8883f4baabdf435fb16a13bff4a40aa2
O=Cc1c[nH]c(-c2ccccc2)c1.O=S(=O)(Cl)c1cccnc1>>O=Cc1cc(-c2ccccc2)n(S(=O)(=O)c2cccnc2)c1
Cl.N1=CC(=CC=C1)S(=O)(=O)Cl.[H-].[Na+].C1(=CC=CC=C1)C1=CC(=CN1)C=O.C1COCCOCCOCCOCCO1>>C1(=CC=CC=C1)C1=CC(=CN1S(=O)(=O)C=1C=NC=CC1)C=O
[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][cH:9][cH:10][cH:11]2)[nH:12][cH:22]1.Cl[S:13](=[O:14])(=[O:15])[c:16]1[cH:17][cH:18][cH:19][n:20][cH:21]1>>[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][cH:9][cH:10][cH:11]2)[n:12]([S:13](=[O:14])(=[O:15])[c:16]2[cH:17][cH:18][cH:19][n:20][cH:21]2)[cH:22]1
O=Cc1c[nH]c(-c2ccccc2)c1.O=S(=O)(Cl)c1cccnc1
O=Cc1cc(-c2ccccc2)n(S(=O)(=O)c2cccnc2)c1
null
null
O1CCCC1.C(C)(=O)OCC
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8].[O;D1;H0:9]=[C:10]-[c:11]1:[c:12]:[nH;D2;+0:13]:[c:14](-[c:15]):[c:16]:1>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8])-[n;H0;D3;+0:13]1:[c:12]:[c:11](-[C:10]=[O;D1;H0:9]):[c:16]:[c:14]:1-[c:15]
75.3
[{"value": 75.0, "product": "C1(=CC=CC=C1)C1=CC(=CN1S(=O)(=O)C=1C=NC=CC1)C=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 75.3, "product": "C1(=CC=CC=C1)C1=CC(=CN1S(=O)(=O)C=1C=NC=CC1)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Under an argon atmosphere, 5-phenyl-1H-pyrrole-3-carbaldehyde (342 mg) was dissolved in absolute tetrahydrofuran (20 mL) and sodium hydride (60% in oil, 240 mg) was added while stirring at room temperature. After stirring at the same temperature for 15 min, 15-crown-5 (1.21 mL) was added, and the mixture was further st...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccccc1.c1ccncc1
HCl
O1CCCC1.C(C)(=O)OCC
null
null
O=Cc1c[nH]c(-c2ccccc2)c1.O=S(=O)(Cl)c1cccnc1>O1CCCC1.C(C)(=O)OCC>O=Cc1cc(-c2ccccc2)n(S(=O)(=O)c2cccnc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0cd100819cde4f4a8f826c6ad1e8d796
COc1ccc(S(=O)(=O)Cl)cn1.O=Cc1c[nH]c(-c2ccccc2)c1>>COc1ccc(S(=O)(=O)n2cc(C=O)cc2-c2ccccc2)cn1
COC1=CC=C(C=N1)S(=O)(=O)Cl.[H-].[Na+].C1(=CC=CC=C1)C1=CC(=CN1)C=O.C1COCCOCCOCCOCCO1>>COC1=CC=C(C=N1)S(=O)(=O)N1C=C(C=C1C1=CC=CC=C1)C=O
Cl[S:7]([c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[n:24][cH:23]1)(=[O:8])=[O:9].[nH:10]1[cH:11][c:12]([CH:13]=[O:14])[cH:15][c:16]1-[c:17]1[cH:18][cH:19][cH:20][cH:21][cH:22]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([S:7](=[O:8])(=[O:9])[n:10]2[cH:11][c:12]([CH:13]=[O:14])[cH:15][c:16]2-[c:17]2[cH:18][cH:19][cH:20][cH:21][cH:2...
COc1ccc(S(=O)(=O)Cl)cn1.O=Cc1c[nH]c(-c2ccccc2)c1
COc1ccc(S(=O)(=O)n2cc(C=O)cc2-c2ccccc2)cn1
null
null
O1CCCC1.C(C)(=O)OCC
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8].[O;D1;H0:9]=[C:10]-[c:11]1:[c:12]:[nH;D2;+0:13]:[c:14](-[c:15]):[c:16]:1>>[O;D1;H0:9]=[C:10]-[c:11]1:[c:12]:[n;H0;D3;+0:13](-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8]):[c:14](-[c:15]):[c:16]:1
17.3
[{"value": 17.0, "product": "COC1=CC=C(C=N1)S(=O)(=O)N1C=C(C=C1C1=CC=CC=C1)C=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 17.3, "product": "COC1=CC=C(C=N1)S(=O)(=O)N1C=C(C=C1C1=CC=CC=C1)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Under an argon atmosphere, 5-phenyl-1H-pyrrole-3-carbaldehyde (171 mg) was dissolved in absolute tetrahydrofuran (20 mL), and sodium hydride (60% in oil, 200 mg) was added at room temperature while stirring. After stirring at the same temperature for 15 min, 15-crown-5 (1.01 mL) was added, and the mixture was further s...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1ccncc1.c1cc[nH]c1.c1ccccc1
HCl
O1CCCC1.C(C)(=O)OCC
null
null
COc1ccc(S(=O)(=O)Cl)cn1.O=Cc1c[nH]c(-c2ccccc2)c1>O1CCCC1.C(C)(=O)OCC>COc1ccc(S(=O)(=O)n2cc(C=O)cc2-c2ccccc2)cn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-02f779fe96b849acbc03beab8e2869c6
O=Cc1c[nH]c(-c2ccccc2)c1.O=S(=O)(Cl)c1ccc(Cl)nc1>>O=Cc1cc(-c2ccccc2)n(S(=O)(=O)c2ccc(Cl)nc2)c1
ClC1=CC=C(C=N1)S(=O)(=O)Cl.[H-].[Na+].C1(=CC=CC=C1)C1=CC(=CN1)C=O.C1COCCOCCOCCOCCO1>>ClC1=CC=C(C=N1)S(=O)(=O)N1C=C(C=C1C1=CC=CC=C1)C=O
[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][cH:9][cH:10][cH:11]2)[nH:12][cH:23]1.Cl[S:13](=[O:14])(=[O:15])[c:16]1[cH:17][cH:18][c:19]([Cl:20])[n:21][cH:22]1>>[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][cH:9][cH:10][cH:11]2)[n:12]([S:13](=[O:14])(=[O:15])[c:16]2[cH:17][cH:18][c:19]([Cl:20])[n:21][cH:22]2)[c...
O=Cc1c[nH]c(-c2ccccc2)c1.O=S(=O)(Cl)c1ccc(Cl)nc1
O=Cc1cc(-c2ccccc2)n(S(=O)(=O)c2ccc(Cl)nc2)c1
null
null
O1CCCC1.C(C)(=O)OCC
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8].[O;D1;H0:9]=[C:10]-[c:11]1:[c:12]:[nH;D2;+0:13]:[c:14](-[c:15]):[c:16]:1>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8])-[n;H0;D3;+0:13]1:[c:12]:[c:11](-[C:10]=[O;D1;H0:9]):[c:16]:[c:14]:1-[c:15]
73.2
[{"value": 73.0, "product": "ClC1=CC=C(C=N1)S(=O)(=O)N1C=C(C=C1C1=CC=CC=C1)C=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 73.2, "product": "ClC1=CC=C(C=N1)S(=O)(=O)N1C=C(C=C1C1=CC=CC=C1)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Under an argon atmosphere, 5-phenyl-1H-pyrrole-3-carbaldehyde (514 mg) was dissolved in absolute tetrahydrofuran (15 mL), and sodium hydride (60% in oil, 180 mg) was added at room temperature while stirring. After stirring at the same temperature for 15 min, 15-crown-5 (0.90 mL) was added, and the mixture was further s...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccccc1.c1ccncc1
HCl
O1CCCC1.C(C)(=O)OCC
null
null
O=Cc1c[nH]c(-c2ccccc2)c1.O=S(=O)(Cl)c1ccc(Cl)nc1>O1CCCC1.C(C)(=O)OCC>O=Cc1cc(-c2ccccc2)n(S(=O)(=O)c2ccc(Cl)nc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6e0b5aee549d487391ae6476f97e5172
O=Cc1c[nH]c(-c2ccccc2)c1.O=S(=O)(Cl)c1cccnc1Cl>>O=Cc1cc(-c2ccccc2)n(S(=O)(=O)c2cccnc2Cl)c1
ClC1=NC=CC=C1S(=O)(=O)Cl.C1(=CC=CC=C1)C1=CC(=CN1)C=O.[H-].[Na+].C1COCCOCCOCCOCCO1>>ClC1=NC=CC=C1S(=O)(=O)N1C=C(C=C1C1=CC=CC=C1)C=O
[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][cH:9][cH:10][cH:11]2)[nH:12][cH:23]1.Cl[S:13](=[O:14])(=[O:15])[c:16]1[cH:17][cH:18][cH:19][n:20][c:21]1[Cl:22]>>[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][cH:9][cH:10][cH:11]2)[n:12]([S:13](=[O:14])(=[O:15])[c:16]2[cH:17][cH:18][cH:19][n:20][c:21]2[Cl:22])[cH:23...
O=Cc1c[nH]c(-c2ccccc2)c1.O=S(=O)(Cl)c1cccnc1Cl
O=Cc1cc(-c2ccccc2)n(S(=O)(=O)c2cccnc2Cl)c1
null
null
null
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6](-[Cl;D1;H0:7]):[#7;a:8]:[c:9].[O;D1;H0:10]=[C:11]-[c:12]1:[c:13]:[nH;D2;+0:14]:[c:15](-[c:16]):[c:17]:1>>[Cl;D1;H0:7]-[c:6](:[#7;a:8]:[c:9]):[c:4](-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[n;H0;D3;+0:14]1:[c:13]:[c:12](-[C:11]=[O;D1;H0:10]):[c:17]:[c:...
null
[]
null
null
null
null
By a reaction under similar conditions as in Reference Example 55 and using 5-phenyl-1H-pyrrole-3-carbaldehyde (514 mg), sodium hydride (60% in oil, 180 mg), 15-crown-5 (0.90 mL) and 2-chloro-3-pyridinesulfonyl chloride (716 mg), the title compound was obtained as an amorphous form (yield 716 mg, 69%). Conditions: See ...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccccc1.c1ccncc1
HCl
null
null
null
O=Cc1c[nH]c(-c2ccccc2)c1.O=S(=O)(Cl)c1cccnc1Cl>>O=Cc1cc(-c2ccccc2)n(S(=O)(=O)c2cccnc2Cl)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-cd5280fdfbd64f9bb1ebe55519466ff3
O=Cc1c[nH]c(-c2ccccc2)c1.O=S(=O)(Cl)c1cnc(Cl)nc1>>O=Cc1cc(-c2ccccc2)n(S(=O)(=O)c2cnc(Cl)nc2)c1
C1COCCOCCOCCOCCO1.C1(=CC=CC=C1)C1=CC(=CN1)C=O.ClC1=NC=C(C=N1)S(=O)(=O)Cl.[H-].[Na+]>>ClC1=NC=C(C=N1)S(=O)(=O)N1C=C(C=C1C1=CC=CC=C1)C=O
[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][cH:9][cH:10][cH:11]2)[nH:12][cH:23]1.Cl[S:13](=[O:14])(=[O:15])[c:16]1[cH:17][n:18][c:19]([Cl:20])[n:21][cH:22]1>>[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][cH:9][cH:10][cH:11]2)[n:12]([S:13](=[O:14])(=[O:15])[c:16]2[cH:17][n:18][c:19]([Cl:20])[n:21][cH:22]2)[cH:...
O=Cc1c[nH]c(-c2ccccc2)c1.O=S(=O)(Cl)c1cnc(Cl)nc1
O=Cc1cc(-c2ccccc2)n(S(=O)(=O)c2cnc(Cl)nc2)c1
null
null
null
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cncnc1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4]1:[c:5]:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:1.[O;D1;H0:10]=[C:11]-[c:12]1:[c:13]:[nH;D2;+0:14]:[c:15](-[c:16]):[c:17]:1>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[c:4]1:[c:5]:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:1)-[n;H0;D3;+0:14]1:[c:13]:[c:12](-[C:11]=[O;D1;H0:10]):[c:17]:[c:15]...
56
[{"value": 56.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a reaction under similar conditions as in Reference Example 55 and using 5-phenyl-1H-pyrrole-3-carbaldehyde (342 mg), sodium hydride (60% in oil, 120 mg), 15-crown-5 (0.60 mL) and 2-chloro-5-pyrimidinesulfonyl chloride (554 mg), the title compound was obtained as a yellow solid (yield 390 mg, 56%). Conditions: See r...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccccc1.c1cncnc1
HCl
null
null
null
O=Cc1c[nH]c(-c2ccccc2)c1.O=S(=O)(Cl)c1cnc(Cl)nc1>>O=Cc1cc(-c2ccccc2)n(S(=O)(=O)c2cnc(Cl)nc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2a78abdc8a174bba9efafa4a8504c9ec
Cc1cc(S(=O)(=O)Cl)cnc1Cl.O=Cc1c[nH]c(-c2ccccc2)c1>>Cc1cc(S(=O)(=O)n2cc(C=O)cc2-c2ccccc2)cnc1Cl
C1COCCOCCOCCOCCO1.C1(=CC=CC=C1)C1=CC(=CN1)C=O.ClC1=C(C=C(C=N1)S(=O)(=O)Cl)C.[H-].[Na+]>>ClC1=C(C=C(C=N1)S(=O)(=O)N1C=C(C=C1C1=CC=CC=C1)C=O)C
Cl[S:5]([c:4]1[cH:3][c:2]([CH3:1])[c:23]([Cl:24])[n:22][cH:21]1)(=[O:6])=[O:7].[nH:8]1[cH:9][c:10]([CH:11]=[O:12])[cH:13][c:14]1-[c:15]1[cH:16][cH:17][cH:18][cH:19][cH:20]1>>[CH3:1][c:2]1[cH:3][c:4]([S:5](=[O:6])(=[O:7])[n:8]2[cH:9][c:10]([CH:11]=[O:12])[cH:13][c:14]2-[c:15]2[cH:16][cH:17][cH:18][cH:19][cH:20]2)[cH:21]...
Cc1cc(S(=O)(=O)Cl)cnc1Cl.O=Cc1c[nH]c(-c2ccccc2)c1
Cc1cc(S(=O)(=O)n2cc(C=O)cc2-c2ccccc2)cnc1Cl
null
null
null
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8].[O;D1;H0:9]=[C:10]-[c:11]1:[c:12]:[c:13](-[c:14]):[nH;D2;+0:15]:[c:16]:1>>[O;D1;H0:9]=[C:10]-[c:11]1:[c:12]:[c:13](-[c:14]):[n;H0;D3;+0:15](-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8]):[c:16]:1
68
[{"value": 68.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a reaction under similar conditions as in Reference Example 55 and using 5-phenyl-1H-pyrrole-3-carbaldehyde (171 mg), sodium hydride (60% in oil, 60 mg), 15-crown-5 (0.30 mL) and 6-chloro-5-methylpyridine-3-sulfonyl chloride (270 mg), the title compound was obtained as a solid (yield 244 mg, 68%). Conditions: See re...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1ccncc1.c1cc[nH]c1.c1ccccc1
HCl
null
null
null
Cc1cc(S(=O)(=O)Cl)cnc1Cl.O=Cc1c[nH]c(-c2ccccc2)c1>>Cc1cc(S(=O)(=O)n2cc(C=O)cc2-c2ccccc2)cnc1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5d2fc4d0769542a1ab87ba3f39834d78
CCOC(=O)c1cc(-c2ccccc2)n(S(=O)(=O)c2cccnc2)c1C>>Cc1c(C=O)cc(-c2ccccc2)n1S(=O)(=O)c1cccnc1
[H-].C(C(C)C)[Al+]CC(C)C.CC=1N(C(=CC1C(=O)OCC)C1=CC=CC=C1)S(=O)(=O)C=1C=NC=CC1.O.C(C)(=O)OCC>>CC=1N(C(=CC1C=O)C1=CC=CC=C1)S(=O)(=O)C=1C=NC=CC1
CCO[C:4]([c:3]1[c:2]([CH3:1])[n:14]([S:15](=[O:16])(=[O:17])[c:18]2[cH:19][cH:20][cH:21][n:22][cH:23]2)[c:7](-[c:8]2[cH:9][cH:10][cH:11][cH:12][cH:13]2)[cH:6]1)=[O:5]>>[CH3:1][c:2]1[c:3]([CH:4]=[O:5])[cH:6][c:7](-[c:8]2[cH:9][cH:10][cH:11][cH:12][cH:13]2)[n:14]1[S:15](=[O:16])(=[O:17])[c:18]1[cH:19][cH:20][cH:21][n:22]...
CCOC(=O)c1cc(-c2ccccc2)n(S(=O)(=O)c2cccnc2)c1C
Cc1c(C=O)cc(-c2ccccc2)n1S(=O)(=O)c1cccnc1
null
null
O1CCCC1.C1(=CC=CC=C1)C
Reduction
OtherReaction
ec1c6c64dd9be73981e5a6c952ab740869d298b20e87e097e88e1179cc5bc6dc
33ddc7b9457742ba0a376f08a972e4f33779267f6f1fe15e3be786427ae9f4ec
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[c:5]:[#7;a:6](-[#16:7]):[c:8]:1-[C;D1;H3:9]>>[#16:7]-[#7;a:6]1:[c:5]:[c:4]:[c:3](-[CH;D2;+0:1]=[O;D1;H0:2]):[c:8]:1-[C;D1;H3:9]
27.2
[{"value": 27.0, "product": "CC=1N(C(=CC1C=O)C1=CC=CC=C1)S(=O)(=O)C=1C=NC=CC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 27.2, "product": "CC=1N(C(=CC1C=O)C1=CC=CC=C1)S(=O)(=O)C=1C=NC=CC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
30
MINUTE
A solution (15 mL) of ethyl 2-methyl-5-phenyl-1-(pyridin-3-ylsulfonyl)-1H-pyrrole-3-carboxylate (980 mg) in tetrahydrofuran was cooled to −78° C., a 1.5 mol/L solution (5.3 mL) of diisobutylaluminum hydride in toluene was added dropwise over 10 min., and the mixture was warmed to 0° C. over 2 hr. Water (100 mL) and eth...
10.6084/m9.figshare.5104873.v1
null
Ester
Aldehyde
null
null
c1c[nH]cc1.c1ccccc1.c1ccncc1
HO-
O1CCCC1.C1(=CC=CC=C1)C
0
0.5
CCOC(=O)c1cc(-c2ccccc2)n(S(=O)(=O)c2cccnc2)c1C>O1CCCC1.C1(=CC=CC=C1)C>Cc1c(C=O)cc(-c2ccccc2)n1S(=O)(=O)c1cccnc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1e56ba46b9794e88b28e4147955ece9c
O=Cc1c[nH]c(-c2ccccc2F)c1.O=S(=O)(Cl)c1cccnc1>>O=Cc1cc(-c2ccccc2F)n(S(=O)(=O)c2cccnc2)c1
Cl.N1=CC(=CC=C1)S(=O)(=O)Cl.C1COCCOCCOCCOCCO1.FC1=C(C=CC=C1)C1=CC(=CN1)C=O.[H-].[Na+]>>FC1=C(C=CC=C1)C1=CC(=CN1S(=O)(=O)C=1C=NC=CC1)C=O
[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][cH:9][cH:10][c:11]2[F:12])[nH:13][cH:23]1.Cl[S:14](=[O:15])(=[O:16])[c:17]1[cH:18][cH:19][cH:20][n:21][cH:22]1>>[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][cH:9][cH:10][c:11]2[F:12])[n:13]([S:14](=[O:15])(=[O:16])[c:17]2[cH:18][cH:19][cH:20][n:21][cH:22]2)[cH:23]1
O=Cc1c[nH]c(-c2ccccc2F)c1.O=S(=O)(Cl)c1cccnc1
O=Cc1cc(-c2ccccc2F)n(S(=O)(=O)c2cccnc2)c1
null
null
O1CCCC1.[Cl-].[Na+].O
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8].[O;D1;H0:9]=[C:10]-[c:11]1:[c:12]:[nH;D2;+0:13]:[c:14](-[c:15]):[c:16]:1>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8])-[n;H0;D3;+0:13]1:[c:12]:[c:11](-[C:10]=[O;D1;H0:9]):[c:16]:[c:14]:1-[c:15]
82
[{"value": 82.0, "product": "FC1=C(C=CC=C1)C1=CC(=CN1S(=O)(=O)C=1C=NC=CC1)C=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 82.0, "product": "FC1=C(C=CC=C1)C1=CC(=CN1S(=O)(=O)C=1C=NC=CC1)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
To a solution (96 mL) of 5-(2-fluorophenyl)-1H-pyrrole-3-carbaldehyde (475 mg) in tetrahydrofuran was added sodium hydride (60% in oil, 503 mg) at room temperature and the mixture was stirred for 30 min. 15-Crown-5 (2.77 g) was added dropwise and the mixture was stirred for 30 min. Pyridine-3-sulfonyl chloride hydrochl...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccccc1.c1ccncc1
HCl
O1CCCC1.[Cl-].[Na+].O
null
0.5
O=Cc1c[nH]c(-c2ccccc2F)c1.O=S(=O)(Cl)c1cccnc1>O1CCCC1.[Cl-].[Na+].O>O=Cc1cc(-c2ccccc2F)n(S(=O)(=O)c2cccnc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9787ac34004545eead5ce2fc3ff2242f
O=Cc1c[nH]c(-c2ccccc2C(F)(F)F)c1.O=S(=O)(Cl)c1cccnc1>>O=Cc1cc(-c2ccccc2C(F)(F)F)n(S(=O)(=O)c2cccnc2)c1
Cl.N1=CC(=CC=C1)S(=O)(=O)Cl.C1COCCOCCOCCOCCO1.FC(C1=C(C=CC=C1)C1=CC(=CN1)C=O)(F)F.[H-].[Na+]>>N1=CC(=CC=C1)S(=O)(=O)N1C=C(C=C1C1=C(C=CC=C1)C(F)(F)F)C=O
[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][cH:9][cH:10][c:11]2[C:12]([F:13])([F:14])[F:15])[nH:16][cH:26]1.Cl[S:17](=[O:18])(=[O:19])[c:20]1[cH:21][cH:22][cH:23][n:24][cH:25]1>>[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][cH:9][cH:10][c:11]2[C:12]([F:13])([F:14])[F:15])[n:16]([S:17](=[O:18])(=[O:19])[c:20]2...
O=Cc1c[nH]c(-c2ccccc2C(F)(F)F)c1.O=S(=O)(Cl)c1cccnc1
O=Cc1cc(-c2ccccc2C(F)(F)F)n(S(=O)(=O)c2cccnc2)c1
null
null
O1CCCC1.[Cl-].[Na+].O
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8].[O;D1;H0:9]=[C:10]-[c:11]1:[c:12]:[nH;D2;+0:13]:[c:14](-[c:15]):[c:16]:1>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8])-[n;H0;D3;+0:13]1:[c:12]:[c:11](-[C:10]=[O;D1;H0:9]):[c:16]:[c:14]:1-[c:15]
100
[{"value": 100.0, "product": "N1=CC(=CC=C1)S(=O)(=O)N1C=C(C=C1C1=C(C=CC=C1)C(F)(F)F)C=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 99.6, "product": "N1=CC(=CC=C1)S(=O)(=O)N1C=C(C=C1C1=C(C=CC=C1)C(F)(F)F)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
To a solution (36 mL) of 5-[2-(trifluoromethyl)phenyl]-1H-pyrrole-3-carbaldehyde (240 mg) in tetrahydrofuran was added sodium hydride (60% in oil, 201 mg) at room temperature and the mixture was stirred for 30 min. 15-Crown-5 (1.11 g) was added dropwise and the mixture was stirred for 30 min. Pyridine-3-sulfonyl chlori...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccccc1.c1ccncc1
HCl
O1CCCC1.[Cl-].[Na+].O
null
0.5
O=Cc1c[nH]c(-c2ccccc2C(F)(F)F)c1.O=S(=O)(Cl)c1cccnc1>O1CCCC1.[Cl-].[Na+].O>O=Cc1cc(-c2ccccc2C(F)(F)F)n(S(=O)(=O)c2cccnc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-46a73add8daf40348c260d6bdccbd28d
Cc1c(C=O)c[nH]c1-c1ccccc1.O=S(=O)(Cl)c1cccnc1>>Cc1c(C=O)cn(S(=O)(=O)c2cccnc2)c1-c1ccccc1
Cl.N1=CC(=CC=C1)S(=O)(=O)Cl.[H-].[Na+].CC=1C(=CNC1C1=CC=CC=C1)C=O.C1COCCOCCOCCOCCO1>>CC=1C(=CN(C1C1=CC=CC=C1)S(=O)(=O)C=1C=NC=CC1)C=O
[CH3:1][c:2]1[c:3]([CH:4]=[O:5])[cH:6][nH:7][c:17]1-[c:18]1[cH:19][cH:20][cH:21][cH:22][cH:23]1.Cl[S:8](=[O:9])(=[O:10])[c:11]1[cH:12][cH:13][cH:14][n:15][cH:16]1>>[CH3:1][c:2]1[c:3]([CH:4]=[O:5])[cH:6][n:7]([S:8](=[O:9])(=[O:10])[c:11]2[cH:12][cH:13][cH:14][n:15][cH:16]2)[c:17]1-[c:18]1[cH:19][cH:20][cH:21][cH:22][cH:...
Cc1c(C=O)c[nH]c1-c1ccccc1.O=S(=O)(Cl)c1cccnc1
Cc1c(C=O)cn(S(=O)(=O)c2cccnc2)c1-c1ccccc1
null
null
O1CCCC1.O
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8].[O;D1;H0:9]=[C:10]-[c:11]1:[c:12]:[c:13](-[c:14]):[nH;D2;+0:15]:[c:16]:1>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8])-[n;H0;D3;+0:15]1:[c:16]:[c:11](-[C:10]=[O;D1;H0:9]):[c:12]:[c:13]:1-[c:14]
53
[{"value": 53.0, "product": "CC=1C(=CN(C1C1=CC=CC=C1)S(=O)(=O)C=1C=NC=CC1)C=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 52.8, "product": "CC=1C(=CN(C1C1=CC=CC=C1)S(=O)(=O)C=1C=NC=CC1)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
4-Methyl-5-phenyl-1H-pyrrole-3-carbaldehyde (185 mg) was dissolved in tetrahydrofuran (10 mL), sodium hydride (60% in oil, 60 mg) was added and the mixture was stirred at room temperature for 15 min. 15-Crown-5 (0.30 mL) was added and the mixture was further stirred at the same temperature for 15 min. 3-Pyridinesulfony...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccncc1.c1ccccc1
HCl
O1CCCC1.O
null
0.25
Cc1c(C=O)c[nH]c1-c1ccccc1.O=S(=O)(Cl)c1cccnc1>O1CCCC1.O>Cc1c(C=O)cn(S(=O)(=O)c2cccnc2)c1-c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-886f6cc7c36942c7934f749e5e49fb9b
Cc1c(C=O)c[nH]c1-c1ccccc1.O=S(=O)(Cl)c1ccccn1>>Cc1c(C=O)cn(S(=O)(=O)c2ccccn2)c1-c1ccccc1
N1=C(C=CC=C1)S(=O)(=O)Cl.CC=1C(=CNC1C1=CC=CC=C1)C=O.[H-].[Na+].C1COCCOCCOCCOCCO1>>CC=1C(=CN(C1C1=CC=CC=C1)S(=O)(=O)C1=NC=CC=C1)C=O
[CH3:1][c:2]1[c:3]([CH:4]=[O:5])[cH:6][nH:7][c:17]1-[c:18]1[cH:19][cH:20][cH:21][cH:22][cH:23]1.Cl[S:8](=[O:9])(=[O:10])[c:11]1[cH:12][cH:13][cH:14][cH:15][n:16]1>>[CH3:1][c:2]1[c:3]([CH:4]=[O:5])[cH:6][n:7]([S:8](=[O:9])(=[O:10])[c:11]2[cH:12][cH:13][cH:14][cH:15][n:16]2)[c:17]1-[c:18]1[cH:19][cH:20][cH:21][cH:22][cH:...
Cc1c(C=O)c[nH]c1-c1ccccc1.O=S(=O)(Cl)c1ccccn1
Cc1c(C=O)cn(S(=O)(=O)c2ccccn2)c1-c1ccccc1
null
null
null
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1ccccn1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[#7;a:6]:[c:7].[O;D1;H0:8]=[C:9]-[c:10]1:[c:11]:[c:12](-[c:13]):[nH;D2;+0:14]:[c:15]:1>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[c:4](:[c:5]):[#7;a:6]:[c:7])-[n;H0;D3;+0:14]1:[c:15]:[c:10](-[C:9]=[O;D1;H0:8]):[c:11]:[c:12]:1-[c:13]
null
[]
null
null
null
null
By a reaction under similar conditions as in Reference Example 65 and using 4-methyl-5-phenyl-1H-pyrrole-3-carbaldehyde (185 mg), sodium hydride (60% in oil, 60 mg), 15-crown-5 (0.30 mL) and 2-pyridinesulfonyl chloride (231 mg) instead of 3-pyridinesulfonyl chloride hydrochloride, the title compound was obtained as an ...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccncc1.c1ccccc1
HCl
null
null
null
Cc1c(C=O)c[nH]c1-c1ccccc1.O=S(=O)(Cl)c1ccccn1>>Cc1c(C=O)cn(S(=O)(=O)c2ccccn2)c1-c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-06fbdbda795c41b9a710b107226f7644
Cc1c(C=O)c[nH]c1-c1ccccc1.Cc1nc(S(=O)(=O)Cl)cn1C>>Cc1c(C=O)cn(S(=O)(=O)c2cn(C)c(C)n2)c1-c1ccccc1
C1COCCOCCOCCOCCO1.CC=1C(=CNC1C1=CC=CC=C1)C=O.CN1C(=NC(=C1)S(=O)(=O)Cl)C.[H-].[Na+]>>CN1C(=NC(=C1)S(=O)(=O)N1C=C(C(=C1C1=CC=CC=C1)C)C=O)C
[CH3:1][c:2]1[c:3]([CH:4]=[O:5])[cH:6][nH:7][c:18]1-[c:19]1[cH:20][cH:21][cH:22][cH:23][cH:24]1.Cl[S:8](=[O:9])(=[O:10])[c:11]1[cH:12][n:13]([CH3:14])[c:15]([CH3:16])[n:17]1>>[CH3:1][c:2]1[c:3]([CH:4]=[O:5])[cH:6][n:7]([S:8](=[O:9])(=[O:10])[c:11]2[cH:12][n:13]([CH3:14])[c:15]([CH3:16])[n:17]2)[c:18]1-[c:19]1[cH:20][cH...
Cc1c(C=O)c[nH]c1-c1ccccc1.Cc1nc(S(=O)(=O)Cl)cn1C
Cc1c(C=O)cn(S(=O)(=O)c2cn(C)c(C)n2)c1-c1ccccc1
null
null
null
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1c[nH]cn1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4]1:[#7;a:5]:[c:6]:[#7;a:7](-[C;D1;H3:8]):[c:9]:1.[O;D1;H0:10]=[C:11]-[c:12]1:[c:13]:[c:14](-[c:15]):[nH;D2;+0:16]:[c:17]:1>>[C;D1;H3:8]-[#7;a:7]1:[c:9]:[c:4](-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[n;H0;D3;+0:16]2:[c:17]:[c:12](-[C:11]=[O;D1;H0:10]):[c:13]:[c:14]:2...
86
[{"value": 86.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a reaction under similar conditions as in Reference Example 65 and using 4-methyl-5-phenyl-1H-pyrrole-3-carbaldehyde (185 mg), sodium hydride (60% in oil, 60 mg), 15-crown-5 (0.30 mL) and (1,2-dimethyl-1H-imidazol-4-yl)sulfonyl chloride (253 mg), the title compound was obtained as a colorless solid (yield 294 mg, 86...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1c[nH]cn1.c1ccccc1
HCl
null
null
null
Cc1c(C=O)c[nH]c1-c1ccccc1.Cc1nc(S(=O)(=O)Cl)cn1C>>Cc1c(C=O)cn(S(=O)(=O)c2cn(C)c(C)n2)c1-c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-eaf0169436754701ae6ff1e949eba783
Cc1c(C=O)c[nH]c1-c1ccccc1.Cc1nn(C)c(Cl)c1S(=O)(=O)Cl>>Cc1nn(C)c(Cl)c1S(=O)(=O)n1cc(C=O)c(C)c1-c1ccccc1
C1COCCOCCOCCOCCO1.CC=1C(=CNC1C1=CC=CC=C1)C=O.ClC1=C(C(=NN1C)C)S(=O)(=O)Cl.[H-].[Na+]>>ClC1=C(C(=NN1C)C)S(=O)(=O)N1C=C(C(=C1C1=CC=CC=C1)C)C=O
[nH:12]1[cH:13][c:14]([CH:15]=[O:16])[c:17]([CH3:18])[c:19]1-[c:20]1[cH:21][cH:22][cH:23][cH:24][cH:25]1.Cl[S:9]([c:8]1[c:2]([CH3:1])[n:3][n:4]([CH3:5])[c:6]1[Cl:7])(=[O:10])=[O:11]>>[CH3:1][c:2]1[n:3][n:4]([CH3:5])[c:6]([Cl:7])[c:8]1[S:9](=[O:10])(=[O:11])[n:12]1[cH:13][c:14]([CH:15]=[O:16])[c:17]([CH3:18])[c:19]1-[c:...
Cc1c(C=O)c[nH]c1-c1ccccc1.Cc1nn(C)c(Cl)c1S(=O)(=O)Cl
Cc1nn(C)c(Cl)c1S(=O)(=O)n1cc(C=O)c(C)c1-c1ccccc1
null
null
null
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cn[nH]c1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4]1:[c:5](-[C;D1;H3:6]):[#7;a:7]:[#7;a:8](-[C;D1;H3:9]):[c:10]:1-[Cl;D1;H0:11].[O;D1;H0:12]=[C:13]-[c:14]1:[c:15]:[nH;D2;+0:16]:[c:17](-[c:18]):[c:19]:1>>[C;D1;H3:6]-[c:5]1:[#7;a:7]:[#7;a:8](-[C;D1;H3:9]):[c:10](-[Cl;D1;H0:11]):[c:4]:1-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1...
100
[{"value": 100.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a reaction under similar conditions as in Reference Example 65 and using 4-methyl-5-phenyl-1H-pyrrole-3-carbaldehyde (185 mg), sodium hydride (60% in oil, 60 mg), 15-crown-5 (0.30 mL) and (5-chloro-1,3-dimethyl-1H-pyrazol-4-yl)sulfonyl chloride (298 mg), the title compound was obtained as an oil (yield 379 mg, about...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cn[nH]c1.c1cc[nH]c1.c1ccccc1
HCl
null
null
null
Cc1c(C=O)c[nH]c1-c1ccccc1.Cc1nn(C)c(Cl)c1S(=O)(=O)Cl>>Cc1nn(C)c(Cl)c1S(=O)(=O)n1cc(C=O)c(C)c1-c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-44a99158ff5c483593a6f5a68a2a423f
Cc1c(C=O)c[nH]c1-c1ccccc1.Cc1nc(C)c(S(=O)(=O)Cl)s1>>Cc1nc(C)c(S(=O)(=O)n2cc(C=O)c(C)c2-c2ccccc2)s1
C1COCCOCCOCCOCCO1.CC=1C(=CNC1C1=CC=CC=C1)C=O.CC=1SC(=C(N1)C)S(=O)(=O)Cl.[H-].[Na+]>>CC=1SC(=C(N1)C)S(=O)(=O)N1C=C(C(=C1C1=CC=CC=C1)C)C=O
[nH:10]1[cH:11][c:12]([CH:13]=[O:14])[c:15]([CH3:16])[c:17]1-[c:18]1[cH:19][cH:20][cH:21][cH:22][cH:23]1.Cl[S:7]([c:6]1[c:4]([CH3:5])[n:3][c:2]([CH3:1])[s:24]1)(=[O:8])=[O:9]>>[CH3:1][c:2]1[n:3][c:4]([CH3:5])[c:6]([S:7](=[O:8])(=[O:9])[n:10]2[cH:11][c:12]([CH:13]=[O:14])[c:15]([CH3:16])[c:17]2-[c:18]2[cH:19][cH:20][cH:...
Cc1c(C=O)c[nH]c1-c1ccccc1.Cc1nc(C)c(S(=O)(=O)Cl)s1
Cc1nc(C)c(S(=O)(=O)n2cc(C=O)c(C)c2-c2ccccc2)s1
null
null
null
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cncs1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4]1:[#16;a:5]:[c:6]:[#7;a:7]:[c:8]:1-[C;D1;H3:9].[O;D1;H0:10]=[C:11]-[c:12]1:[c:13]:[nH;D2;+0:14]:[c:15](-[c:16]):[c:17]:1>>[C;D1;H3:9]-[c:8]1:[#7;a:7]:[c:6]:[#16;a:5]:[c:4]:1-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[n;H0;D3;+0:14]1:[c:13]:[c:12](-[C:11]=[O;D1;H0:10])...
8
[{"value": 8.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a reaction under similar conditions as in Reference Example 65 and using 4-methyl-5-phenyl-1H-pyrrole-3-carbaldehyde (185 mg), sodium hydride (60% in oil, 60 mg), 15-crown-5 (0.30 mL) and (2,4-dimethyl-1,3-thiazol-5-yl)sulfonyl chloride (275 mg), the title compound was obtained as an oil (yield 27.8 mg, 8%). Conditi...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cscn1.c1cc[nH]c1.c1ccccc1
HCl
null
null
null
Cc1c(C=O)c[nH]c1-c1ccccc1.Cc1nc(C)c(S(=O)(=O)Cl)s1>>Cc1nc(C)c(S(=O)(=O)n2cc(C=O)c(C)c2-c2ccccc2)s1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2f83347bc4d04a07bf983a37be4c26a8
Cc1c(C=O)c[nH]c1-c1ccccc1F.O=S(=O)(Cl)c1cccnc1>>Cc1c(C=O)cn(S(=O)(=O)c2cccnc2)c1-c1ccccc1F
C1COCCOCCOCCOCCO1.FC1=C(C=CC=C1)C1=C(C(=CN1)C=O)C.Cl.N1=CC(=CC=C1)S(=O)(=O)Cl.[H-].[Na+]>>FC1=C(C=CC=C1)C1=C(C(=CN1S(=O)(=O)C=1C=NC=CC1)C=O)C
[CH3:1][c:2]1[c:3]([CH:4]=[O:5])[cH:6][nH:7][c:17]1-[c:18]1[cH:19][cH:20][cH:21][cH:22][c:23]1[F:24].Cl[S:8](=[O:9])(=[O:10])[c:11]1[cH:12][cH:13][cH:14][n:15][cH:16]1>>[CH3:1][c:2]1[c:3]([CH:4]=[O:5])[cH:6][n:7]([S:8](=[O:9])(=[O:10])[c:11]2[cH:12][cH:13][cH:14][n:15][cH:16]2)[c:17]1-[c:18]1[cH:19][cH:20][cH:21][cH:22...
Cc1c(C=O)c[nH]c1-c1ccccc1F.O=S(=O)(Cl)c1cccnc1
Cc1c(C=O)cn(S(=O)(=O)c2cccnc2)c1-c1ccccc1F
null
null
null
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8].[O;D1;H0:9]=[C:10]-[c:11]1:[c:12]:[c:13](-[c:14]):[nH;D2;+0:15]:[c:16]:1>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8])-[n;H0;D3;+0:15]1:[c:16]:[c:11](-[C:10]=[O;D1;H0:9]):[c:12]:[c:13]:1-[c:14]
87
[{"value": 87.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a similar operation as in Reference Example 65 and using 5-(2-fluorophenyl)-4-methyl-1H-pyrrole-3-carbaldehyde (301 mg), sodium hydride (60% in oil, 179 mg), 15-crown-5 (0.88 mL) and pyridin-3-ylsulfonyl chloride hydrochloride (476 mg), the title compound was obtained as white crystals (yield 440 mg, 87%). Condition...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccncc1.c1ccccc1
HCl
null
null
null
Cc1c(C=O)c[nH]c1-c1ccccc1F.O=S(=O)(Cl)c1cccnc1>>Cc1c(C=O)cn(S(=O)(=O)c2cccnc2)c1-c1ccccc1F
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7cb62c60d9c9462399bccfcb0b15408b
C[NH3+].O=Cc1cc(Br)n(S(=O)(=O)c2ccccc2)c1>>CNCc1cc(Br)n(S(=O)(=O)c2ccccc2)c1
BrC1=CC(=CN1S(=O)(=O)C1=CC=CC=C1)C=O.[Cl-].C[NH3+].C(#N)[BH3-].[Na+]>>BrC1=CC(=CN1S(=O)(=O)C1=CC=CC=C1)CNC
[CH3:1][NH3+:2].O=[CH:3][c:4]1[cH:5][c:6]([Br:7])[n:8]([S:9](=[O:10])(=[O:11])[c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[cH:18]1>>[CH3:1][NH:2][CH2:3][c:4]1[cH:5][c:6]([Br:7])[n:8]([S:9](=[O:10])(=[O:11])[c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[cH:18]1
C[NH3+].O=Cc1cc(Br)n(S(=O)(=O)c2ccccc2)c1
CNCc1cc(Br)n(S(=O)(=O)c2ccccc2)c1
null
null
CO
Functional Group Interconversion
OtherReaction
f81a06fd4802217f2a89af56ed399b3c54f571141190aacbc8b18232a7f009a7
48e9cfa1233c86fcd1dbe33bcccd5760ec96958bf94448cbcdabe7d9b5e5da4f
O=S(=O)(c1ccccc1)n1cccc1
O=[CH;D2;+0:1]-[c:2]1:[c:3]:[#7;a:4](-[#16:5]):[c:6]:[c:7]:1.[C;D1;H3:8]-[NH3+;D1:9]>>[#16:5]-[#7;a:4]1:[c:3]:[c:2](-[CH2;D2;+0:1]-[NH;D2;+0:9]-[C;D1;H3:8]):[c:7]:[c:6]:1
120
[{"value": 100.0, "product": "BrC1=CC(=CN1S(=O)(=O)C1=CC=CC=C1)CNC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 120.0, "product": "BrC1=CC(=CN1S(=O)(=O)C1=CC=CC=C1)CNC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a solution (60 mL) of 5-bromo-1-(phenylsulfonyl)-1H-pyrrole-3-carbaldehyde (3.5 g) in methanol were added methylammonium chloride (7.5 g) and sodium cyanoborohydride (2.4 g), and the mixture was stirred at room temperature for 1 hr. The reaction mixture was concentrated under reduced pressure, saturated aqueous sodi...
10.6084/m9.figshare.5104873.v1
null
Aldehyde
Secondary amine
null
null
c1cc[nH]c1.c1ccccc1
HO-
CO
null
1
C[NH3+].O=Cc1cc(Br)n(S(=O)(=O)c2ccccc2)c1>CO>CNCc1cc(Br)n(S(=O)(=O)c2ccccc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7911fa11974844c9a7a009b142ef8d80
CNCc1cc(Br)n(S(=O)(=O)c2ccccc2)c1.O=C([O-])O>>CN(Cc1cc(Br)n(S(=O)(=O)c2ccccc2)c1)C(=O)OC(C)(C)C
C(O)([O-])=O.[Na+].BrC1=CC(=CN1S(=O)(=O)C1=CC=CC=C1)CNC>>C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)Br)S(=O)(=O)C1=CC=CC=C1)=O
[CH3:1][NH:2][CH2:3][c:4]1[cH:5][c:6]([Br:7])[n:8]([S:9](=[O:10])(=[O:11])[c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[cH:18]1.[O-][C:19](=[O:20])[OH:21]>>[CH3:1][N:2]([CH2:3][c:4]1[cH:5][c:6]([Br:7])[n:8]([S:9](=[O:10])(=[O:11])[c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[cH:18]1)[C:19](=[O:20])[O:21][C:22]([CH3:23])(...
CNCc1cc(Br)n(S(=O)(=O)c2ccccc2)c1.O=C([O-])O
CN(Cc1cc(Br)n(S(=O)(=O)c2ccccc2)c1)C(=O)OC(C)(C)C
null
null
C(C)(=O)OCC
C-C Coupling
OtherReaction
b60b7050648178cf87b8461a52efebd4094992e5bd847fac6aeeffea3f185375
ed7cb4f05cf8979caa75e907f8c2b6171bb335392280c8fdecfa71b6334016ad
O=S(=O)(c1ccccc1)n1cccc1
[#7;a:1]:[c:2]:[c:3]-[C:4]-[NH;D2;+0:5]-[C;D1;H3:6].[O-]-[C;H0;D3;+0:7](=[O;D1;H0:8])-[OH;D1;+0:9]>>[#7;a:1]:[c:2]:[c:3]-[C:4]-[N;H0;D3;+0:5](-[C;D1;H3:6])-[C;H0;D3;+0:7](=[O;D1;H0:8])-[O;H0;D2;+0:9]-[C:10](-[C;D1;H3:11])(-[C;D1;H3:12])-[C;D1;H3:13]
73
[{"value": 73.0, "product": "C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)Br)S(=O)(=O)C1=CC=CC=C1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
14
HOUR
To a solution of 1-[5-bromo-1-(phenylsulfonyl)-1H-pyrrol-3-yl]-N-methylmethanamine (4.4 g) in ethyl acetate (60 mL) was added di-tert-butyl bicarbonate (2.8 mL), and the mixture was stirred at room temperature for 14 hr. Saturated aqueous sodium hydrogencarbonate solution was added to the reaction mixture, and the mixt...
10.6084/m9.figshare.5104873.v1
null
Carbonic Acid.Secondary amine
Carbamic ester.Ether.Boc
null
null
c1cc[nH]c1.c1ccccc1
null
C(C)(=O)OCC
null
14
CNCc1cc(Br)n(S(=O)(=O)c2ccccc2)c1.O=C([O-])O>C(C)(=O)OCC>CN(Cc1cc(Br)n(S(=O)(=O)c2ccccc2)c1)C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-838fdcdfc61a45edba58328afeb5994b
CN(Cc1cc(Br)n(S(=O)(=O)c2ccccc2)c1)C(=O)OC(C)(C)C>>CN(Cc1c[nH]c(Br)c1)C(=O)OC(C)(C)C
C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)Br)S(=O)(=O)C1=CC=CC=C1)=O.O>>C(C)(C)(C)OC(N(C)CC1=CNC(=C1)Br)=O
O=S(=O)(c1ccccc1)[n:6]1[cH:5][c:4]([CH2:3][N:2]([CH3:1])[C:10](=[O:11])[O:12][C:13]([CH3:14])([CH3:15])[CH3:16])[cH:9][c:7]1[Br:8]>>[CH3:1][N:2]([CH2:3][c:4]1[cH:5][nH:6][c:7]([Br:8])[cH:9]1)[C:10](=[O:11])[O:12][C:13]([CH3:14])([CH3:15])[CH3:16]
CN(Cc1cc(Br)n(S(=O)(=O)c2ccccc2)c1)C(=O)OC(C)(C)C
CN(Cc1c[nH]c(Br)c1)C(=O)OC(C)(C)C
null
null
O1CCCC1.CO.[OH-].[Na+]
Reduction
OtherReaction
e84bce0a3684cb001278a9df3f54235c2ecd212d7bfeaa59bdd53379604bae1d
312e9350dcad67590617294c0eb017edf0b9fbfe6133c06a3f393b871a889092
c1cc[nH]c1
O=S(=O)(-[n;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[c:5]:1-[Br;D1;H0:6])-c1:c:c:c:c:c:1>>[Br;D1;H0:6]-[c:5]1:[c:4]:[c:3]:[c:2]:[nH;D2;+0:1]:1
61
[{"value": 61.0, "product": "C(C)(C)(C)OC(N(C)CC1=CNC(=C1)Br)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 60.9, "product": "C(C)(C)(C)OC(N(C)CC1=CNC(=C1)Br)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
tert-Butyl{[5-bromo-1-(phenylsulfonyl)-1H-pyrrol-3-yl]methyl}methylcarbamate (1.0 g) was dissolved in a mixed solvent of tetrahydrofuran (15 mL) and methanol (5 mL), and 8 mol/L aqueous sodium hydroxide solution (1.5 mL) was added dropwise at not more than 10° C. After stirring at the same temperature for 4 hr, water w...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ccccc1.c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1
HO-
O1CCCC1.CO.[OH-].[Na+]
null
4
CN(Cc1cc(Br)n(S(=O)(=O)c2ccccc2)c1)C(=O)OC(C)(C)C>O1CCCC1.CO.[OH-].[Na+]>CN(Cc1c[nH]c(Br)c1)C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3f567915120c41ecac6c3480e343b4f5
CN(Cc1c[nH]c(Br)c1)C(=O)OC(C)(C)C.O=S(=O)(Cl)c1cccnc1>>CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
[H-].[Na+].C(C)(C)(C)OC(N(C)CC1=CNC(=C1)Br)=O.C1COCCOCCOCCOCCO1.Cl.N1=CC(=CC=C1)S(=O)(=O)Cl>>C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)Br)S(=O)(=O)C=1C=NC=CC1)=O
[CH3:1][N:2]([CH2:3][c:4]1[cH:5][c:6]([Br:7])[nH:8][cH:18]1)[C:19](=[O:20])[O:21][C:22]([CH3:23])([CH3:24])[CH3:25].Cl[S:9](=[O:10])(=[O:11])[c:12]1[cH:13][cH:14][cH:15][n:16][cH:17]1>>[CH3:1][N:2]([CH2:3][c:4]1[cH:5][c:6]([Br:7])[n:8]([S:9](=[O:10])(=[O:11])[c:12]2[cH:13][cH:14][cH:15][n:16][cH:17]2)[cH:18]1)[C:19](=[...
CN(Cc1c[nH]c(Br)c1)C(=O)OC(C)(C)C.O=S(=O)(Cl)c1cccnc1
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
null
null
O1CCCC1.O.CN(C=O)C
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cccnc1)n1cccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8].[Br;D1;H0:9]-[c:10]1:[c:11]:[c:12]:[c:13]:[nH;D2;+0:14]:1>>[Br;D1;H0:9]-[c:10]1:[c:11]:[c:12]:[c:13]:[n;H0;D3;+0:14]:1-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8]
85.6
[{"value": 85.0, "product": "C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)Br)S(=O)(=O)C=1C=NC=CC1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 85.6, "product": "C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)Br)S(=O)(=O)C=1C=NC=CC1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
To a suspension (10 mL) of sodium hydride (60% in oil, 204 mg) in tetrahydrofuran was added a solution (3 mL) of tert-butyl[(5-bromo-1H-pyrrol-3-yl)methyl]methylcarbamate (410 mg) in N,N-dimethylformamide at 0° C., and 15-crown-5 (938 mg) and pyridin-3-ylsulfonyl chloride hydrochloride (456 mg) were added at the same t...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccncc1
HCl
O1CCCC1.O.CN(C=O)C
null
2
CN(Cc1c[nH]c(Br)c1)C(=O)OC(C)(C)C.O=S(=O)(Cl)c1cccnc1>O1CCCC1.O.CN(C=O)C>CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-eeaa97d24a5346f09f7478792a7aca8a
CN.Cc1cc(S(=O)(=O)n2cc(C=O)cc2-c2ccccc2)cnc1Cl.O=C([O-])O>>Cc1cc(S(=O)(=O)n2cc(CN(C)C(=O)OC(C)(C)C)cc2-c2ccccc2)cnc1Cl
C(O)([O-])=O.[Na+].CN.[BH4-].[Na+].ClC1=C(C=C(C=N1)S(=O)(=O)N1C=C(C=C1C1=CC=CC=C1)C=O)C>>C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)C1=CC=CC=C1)S(=O)(=O)C=1C=NC(=C(C1)C)Cl)=O
[NH2:12][CH3:13].O=[CH:11][c:10]1[cH:9][n:8]([S:5]([c:4]2[cH:3][c:2]([CH3:1])[c:31]([Cl:32])[n:30][cH:29]2)(=[O:6])=[O:7])[c:22](-[c:23]2[cH:24][cH:25][cH:26][cH:17][cH:28]2)[cH:21]1.[O-][C:14](=[O:15])[OH:16]>>[CH3:1][c:2]1[cH:3][c:4]([S:5](=[O:6])(=[O:7])[n:8]2[cH:9][c:10]([CH2:11][N:12]([CH3:13])[C:14](=[O:15])[O:16...
CN.Cc1cc(S(=O)(=O)n2cc(C=O)cc2-c2ccccc2)cnc1Cl.O=C([O-])O
Cc1cc(S(=O)(=O)n2cc(CN(C)C(=O)OC(C)(C)C)cc2-c2ccccc2)cnc1Cl
null
null
O1CCCC1.O.CO
C-C Coupling
OtherReaction
3b707e34799ac6851d60bdaa66c51532260299fc603a1d0d55ae2ba7ff1616a1
3d8ce2b92b61290a79a351e04280a781726e579e49920cac71c26ad6abac8497
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
O=[CH;D2;+0:1]-[c:2]1:[c:3]:[c:4](-[c:5]2:[c:6]:[c:7]:[cH;D2;+0:8]:[cH;D2;+0:9]:[cH;D2;+0:10]:2):[#7;a:11](-[#16:12]):[c:13]:1.[C;D1;H3:14]-[NH2;D1;+0:15].[O-]-[C;H0;D3;+0:16](=[O;D1;H0:17])-[OH;D1;+0:18]>>[#16:12]-[#7;a:11]1:[c:13]:[c:2](-[CH2;D2;+0:1]-[N;H0;D3;+0:15](-[C;D1;H3:14])-[C;H0;D3;+0:16](=[O;D1;H0:17])-[O;H...
77
[{"value": 77.0, "product": "C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)C1=CC=CC=C1)S(=O)(=O)C=1C=NC(=C(C1)C)Cl)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
1-[(6-Chloro-5-methylpyridin-3-yl)sulfonyl]-5-phenyl-1H-pyrrole-3-carbaldehyde (244 mg) was dissolved in absolute tetrahydrofuran (6.8 mL), a 2 mol/L solution (0.34 mL) of methylamine in tetrahydrofuran was added, and the mixture was stirred at room temperature for 4 hr. The reaction mixture was added to a solution of ...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Carbonic Acid.Primary amine
Carbamic ester.Ether.Boc
c1ccccc1
c1ccccc1
c1ccncc1.c1cc[nH]c1.c1ccccc1
null
O1CCCC1.O.CO
null
4
CN.Cc1cc(S(=O)(=O)n2cc(C=O)cc2-c2ccccc2)cnc1Cl.O=C([O-])O>O1CCCC1.O.CO>Cc1cc(S(=O)(=O)n2cc(CN(C)C(=O)OC(C)(C)C)cc2-c2ccccc2)cnc1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b2b7ee5d4bb54cf1a931f04cc07087a8
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.OB(O)c1ccsc1>>CN(Cc1cc(-c2ccsc2)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
BrC1=CC(=CN1S(=O)(=O)C=1C=NC=CC1)CN(C(OC(C)(C)C)=O)C.S1C=C(C=C1)B(O)O.C([O-])([O-])=O.[Na+].[Na+]>>CN(C(OC(C)(C)C)=O)CC1=CN(C(=C1)C1=CSC=C1)S(=O)(=O)C=1C=NC=CC1
Br[c:6]1[cH:5][c:4]([CH2:3][N:2]([CH3:1])[C:23](=[O:24])[O:25][C:26]([CH3:27])([CH3:28])[CH3:29])[cH:22][n:12]1[S:13](=[O:14])(=[O:15])[c:16]1[cH:17][cH:18][cH:19][n:20][cH:21]1.OB(O)[c:7]1[cH:8][cH:9][s:10][cH:11]1>>[CH3:1][N:2]([CH2:3][c:4]1[cH:5][c:6](-[c:7]2[cH:8][cH:9][s:10][cH:11]2)[n:12]([S:13](=[O:14])(=[O:15])...
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.OB(O)c1ccsc1
CN(Cc1cc(-c2ccsc2)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.COCCOC
C-C Coupling
Suzuki coupling with boronic acids
487361cf9c8a098c20bfd7c2c5754120927e29e3849a70b2ee791c6972a05de5
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=S(=O)(c1cccnc1)n1cccc1-c1ccsc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[#7;a:5]:1-[#16:6].O-B(-O)-[c;H0;D3;+0:7]1:[c:8]:[#16;a:9]:[c:10]:[c:11]:1>>[#16:6]-[#7;a:5]1:[c:4]:[c:3]:[c:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:7]1:[c:8]:[#16;a:9]:[c:10]:[c:11]:1
81
[{"value": 81.0, "product": "CN(C(OC(C)(C)C)=O)CC1=CN(C(=C1)C1=CSC=C1)S(=O)(=O)C=1C=NC=CC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 80.9, "product": "CN(C(OC(C)(C)C)=O)CC1=CN(C(=C1)C1=CSC=C1)S(=O)(=O)C=1C=NC=CC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
105
CELSIUS
1
HOUR
Under an argon atmosphere, a suspension of tert-butyl {[5-bromo-1-(pyridin-3-ylsulfonyl)-1H-pyrrol-3-yl]methyl}methylcarbamate (232 mg), 3-thienylboronic acid (138 mg), tetrakis(triphenylphosphine)palladium (31.3 mg) and sodium carbonate (175 mg) in 1,2-dimethoxyethane (10 mL) and water (5 mL) was stirred at 105° C. fo...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1cc[nH]c1.c1ccsc1
c1cc[nH]c1.c1ccsc1
c1cc[nH]c1.c1ccsc1.c1ccncc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC
105
1
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.OB(O)c1ccsc1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC>CN(Cc1cc(-c2ccsc2)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f60495c664e94c12b0a0e88622c77c5c
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.Cc1ccccc1B(O)O>>Cc1ccccc1-c1cc(CN(C)C(=O)OC(C)(C)C)cn1S(=O)(=O)c1cccnc1
C([O-])([O-])=O.[Na+].[Na+].BrC1=CC(=CN1S(=O)(=O)C=1C=NC=CC1)CN(C(OC(C)(C)C)=O)C.CC1=C(C=CC=C1)B(O)O>>CN(C(OC(C)(C)C)=O)CC1=CN(C(=C1)C1=C(C=CC=C1)C)S(=O)(=O)C=1C=NC=CC1
Br[c:8]1[cH:9][c:10]([CH2:11][N:12]([CH3:13])[C:14](=[O:15])[O:16][C:17]([CH3:18])([CH3:19])[CH3:20])[cH:21][n:22]1[S:23](=[O:24])(=[O:25])[c:26]1[cH:27][cH:28][cH:29][n:30][cH:31]1.OB(O)[c:7]1[c:2]([CH3:1])[cH:3][cH:4][cH:5][cH:6]1>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1-[c:8]1[cH:9][c:10]([CH2:11][N:12]([CH3:13]...
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.Cc1ccccc1B(O)O
Cc1ccccc1-c1cc(CN(C)C(=O)OC(C)(C)C)cn1S(=O)(=O)c1cccnc1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
null
C-C Coupling
Suzuki coupling with boronic acids
b71c1accb23fcf6e808cbf7fdd27a50d721fbf67e253875213e991e29cdecd2f
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[#7;a:5]:1-[#16:6].O-B(-O)-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10](-[C;D1;H3:11]):[c:12]>>[#16:6]-[#7;a:5]1:[c:4]:[c:3]:[c:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10](-[C;D1;H3:11]):[c:12]
68
[{"value": 68.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a similar operation as in Reference Example 79 and using tert-butyl {[5-bromo-1-(pyridin-3-ylsulfonyl)-1H-pyrrol-3-yl]methyl}methylcarbamate (300 mg), (2-methylphenyl)boronic acid (190 mg), tetrakis(triphenylphosphine)palladium (40 mg) and sodium carbonate (222 mg), the title compound was obtained as a pale-yellow o...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1cc[nH]c1.c1ccccc1
c1ccccc1.c1cc[nH]c1
c1ccccc1.c1cc[nH]c1.c1ccncc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
null
null
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.Cc1ccccc1B(O)O>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1>Cc1ccccc1-c1cc(CN(C)C(=O)OC(C)(C)C)cn1S(=O)(=O)c1cccnc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1fc61714612e45bb8256116c5181e5ee
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.Cc1ccccc1B(O)O>>Cc1ccccc1-c1cc(CN(C)C(=O)OC(C)(C)C)cn1S(=O)(=O)c1cccnc1
C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)Br)S(=O)(=O)C=1C=NC=CC1)=O.CC1=C(C=CC=C1)B(O)O.C([O-])([O-])=O.[Na+].[Na+]>>CN(C(OC(C)(C)C)=O)CC1=CN(C(=C1)C1=C(C=CC=C1)C)S(=O)(=O)C=1C=NC=CC1
Br[c:8]1[cH:9][c:10]([CH2:11][N:12]([CH3:13])[C:14](=[O:15])[O:16][C:17]([CH3:18])([CH3:19])[CH3:20])[cH:21][n:22]1[S:23](=[O:24])(=[O:25])[c:26]1[cH:27][cH:28][cH:29][n:30][cH:31]1.OB(O)[c:7]1[c:2]([CH3:1])[cH:3][cH:4][cH:5][cH:6]1>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1-[c:8]1[cH:9][c:10]([CH2:11][N:12]([CH3:13]...
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.Cc1ccccc1B(O)O
Cc1ccccc1-c1cc(CN(C)C(=O)OC(C)(C)C)cn1S(=O)(=O)c1cccnc1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.COCCOC
C-C Coupling
Suzuki coupling with boronic acids
b71c1accb23fcf6e808cbf7fdd27a50d721fbf67e253875213e991e29cdecd2f
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[#7;a:5]:1-[#16:6].O-B(-O)-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10](-[C;D1;H3:11]):[c:12]>>[#16:6]-[#7;a:5]1:[c:4]:[c:3]:[c:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10](-[C;D1;H3:11]):[c:12]
68.2
[{"value": 68.0, "product": "CN(C(OC(C)(C)C)=O)CC1=CN(C(=C1)C1=C(C=CC=C1)C)S(=O)(=O)C=1C=NC=CC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 68.2, "product": "CN(C(OC(C)(C)C)=O)CC1=CN(C(=C1)C1=C(C=CC=C1)C)S(=O)(=O)C=1C=NC=CC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
105
CELSIUS
18
HOUR
By a similar operation as in Reference Example 79 and using tert-butyl {[5-bromo-1-(pyridin-3-ylsulfonyl)-1H-pyrrol-3-yl]methyl}methylcarbamate (300 mg), (2-methylphenyl)boronic acid (190 mg), tetrakis(triphenylphosphine)palladium (40 mg) and sodium carbonate (222 mg), the title compound was obtained as a pale-yellow o...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1cc[nH]c1.c1ccccc1
c1ccccc1.c1cc[nH]c1
c1ccccc1.c1cc[nH]c1.c1ccncc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC
105
18
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.Cc1ccccc1B(O)O>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC>Cc1ccccc1-c1cc(CN(C)C(=O)OC(C)(C)C)cn1S(=O)(=O)c1cccnc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-729bc652f32b40d28d6d8220e77c1f60
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.Cc1cc(F)ccc1B(O)O>>Cc1cc(F)ccc1-c1cc(CN(C)C(=O)OC(C)(C)C)cn1S(=O)(=O)c1cccnc1
C([O-])([O-])=O.[Na+].[Na+].C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)Br)S(=O)(=O)C=1C=NC=CC1)=O.FC1=CC(=C(C=C1)B(O)O)C>>C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)C1=C(C=C(C=C1)F)C)S(=O)(=O)C=1C=NC=CC1)=O
Br[c:9]1[cH:10][c:11]([CH2:12][N:13]([CH3:14])[C:15](=[O:16])[O:17][C:18]([CH3:19])([CH3:20])[CH3:21])[cH:22][n:23]1[S:24](=[O:25])(=[O:26])[c:27]1[cH:28][cH:29][cH:30][n:31][cH:32]1.OB(O)[c:8]1[c:2]([CH3:1])[cH:3][c:4]([F:5])[cH:6][cH:7]1>>[CH3:1][c:2]1[cH:3][c:4]([F:5])[cH:6][cH:7][c:8]1-[c:9]1[cH:10][c:11]([CH2:12][...
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.Cc1cc(F)ccc1B(O)O
Cc1cc(F)ccc1-c1cc(CN(C)C(=O)OC(C)(C)C)cn1S(=O)(=O)c1cccnc1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
null
C-C Coupling
Suzuki coupling with boronic acids
b71c1accb23fcf6e808cbf7fdd27a50d721fbf67e253875213e991e29cdecd2f
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[#7;a:5]:1-[#16:6].O-B(-O)-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10](-[C;D1;H3:11]):[c:12]>>[#16:6]-[#7;a:5]1:[c:4]:[c:3]:[c:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10](-[C;D1;H3:11]):[c:12]
67
[{"value": 67.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a similar operation as in Reference Example 79 and using tert-butyl{[5-bromo-1-(pyridin-3-ylsulfonyl)-1H-pyrrol-3-yl]methyl}methylcarbamate (300 mg), (4-fluoro-2-methylphenyl)boronic acid (215 mg), tetrakis(triphenylphosphine)palladium (40 mg) and sodium carbonate (222 mg), the title compound was obtained as a pale-...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1cc[nH]c1.c1ccccc1
c1ccccc1.c1cc[nH]c1
c1ccccc1.c1cc[nH]c1.c1ccncc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
null
null
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.Cc1cc(F)ccc1B(O)O>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1>Cc1cc(F)ccc1-c1cc(CN(C)C(=O)OC(C)(C)C)cn1S(=O)(=O)c1cccnc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-aa5c5ab6a9f841d3b3524f6130d63ef1
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.Cc1cscc1B(O)O>>Cc1cscc1-c1cc(CN(C)C(=O)OC(C)(C)C)cn1S(=O)(=O)c1cccnc1
C([O-])([O-])=O.[Na+].[Na+].C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)Br)S(=O)(=O)C=1C=NC=CC1)=O.CC=1C(=CSC1)B(O)O>>CN(C(OC(C)(C)C)=O)CC1=CN(C(=C1)C1=CSC=C1C)S(=O)(=O)C=1C=NC=CC1
Br[c:7]1[cH:8][c:9]([CH2:10][N:11]([CH3:12])[C:13](=[O:14])[O:15][C:16]([CH3:17])([CH3:18])[CH3:19])[cH:20][n:21]1[S:22](=[O:23])(=[O:24])[c:25]1[cH:26][cH:27][cH:28][n:29][cH:30]1.OB(O)[c:6]1[c:2]([CH3:1])[cH:3][s:4][cH:5]1>>[CH3:1][c:2]1[cH:3][s:4][cH:5][c:6]1-[c:7]1[cH:8][c:9]([CH2:10][N:11]([CH3:12])[C:13](=[O:14])...
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.Cc1cscc1B(O)O
Cc1cscc1-c1cc(CN(C)C(=O)OC(C)(C)C)cn1S(=O)(=O)c1cccnc1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
null
C-C Coupling
Suzuki coupling with boronic acids
487361cf9c8a098c20bfd7c2c5754120927e29e3849a70b2ee791c6972a05de5
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=S(=O)(c1cccnc1)n1cccc1-c1ccsc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[#7;a:5]:1-[#16:6].O-B(-O)-[c;H0;D3;+0:7]1:[c:8]:[#16;a:9]:[c:10]:[c:11]:1-[C;D1;H3:12]>>[#16:6]-[#7;a:5]1:[c:4]:[c:3]:[c:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:7]1:[c:8]:[#16;a:9]:[c:10]:[c:11]:1-[C;D1;H3:12]
64
[{"value": 64.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a similar operation as in Reference Example 79 and using tert-butyl{[5-bromo-1-(pyridin-3-ylsulfonyl)-1H-pyrrol-3-yl]methyl}methylcarbamate (300 mg), (4-methyl-3-thienyl)boronic acid (198 mg), tetrakis(triphenylphosphine)palladium (40 mg) and sodium carbonate (222 mg), the title compound was obtained as a pale-yello...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1cc[nH]c1.c1ccsc1
c1ccsc1.c1cc[nH]c1
c1ccsc1.c1cc[nH]c1.c1ccncc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
null
null
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.Cc1cscc1B(O)O>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1>Cc1cscc1-c1cc(CN(C)C(=O)OC(C)(C)C)cn1S(=O)(=O)c1cccnc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0f683e154a2647dab4297b40fba6bd97
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.Cc1cscc1B(O)O>>Cc1cscc1-c1cc(CN(C)C(=O)OC(C)(C)C)cn1S(=O)(=O)c1cccnc1
C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)Br)S(=O)(=O)C=1C=NC=CC1)=O.CC=1C(=CSC1)B(O)O.C([O-])([O-])=O.[Na+].[Na+]>>CN(C(OC(C)(C)C)=O)CC1=CN(C(=C1)C1=CSC=C1C)S(=O)(=O)C=1C=NC=CC1
Br[c:7]1[cH:8][c:9]([CH2:10][N:11]([CH3:12])[C:13](=[O:14])[O:15][C:16]([CH3:17])([CH3:18])[CH3:19])[cH:20][n:21]1[S:22](=[O:23])(=[O:24])[c:25]1[cH:26][cH:27][cH:28][n:29][cH:30]1.OB(O)[c:6]1[c:2]([CH3:1])[cH:3][s:4][cH:5]1>>[CH3:1][c:2]1[cH:3][s:4][cH:5][c:6]1-[c:7]1[cH:8][c:9]([CH2:10][N:11]([CH3:12])[C:13](=[O:14])...
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.Cc1cscc1B(O)O
Cc1cscc1-c1cc(CN(C)C(=O)OC(C)(C)C)cn1S(=O)(=O)c1cccnc1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.COCCOC
C-C Coupling
Suzuki coupling with boronic acids
487361cf9c8a098c20bfd7c2c5754120927e29e3849a70b2ee791c6972a05de5
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=S(=O)(c1cccnc1)n1cccc1-c1ccsc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[#7;a:5]:1-[#16:6].O-B(-O)-[c;H0;D3;+0:7]1:[c:8]:[#16;a:9]:[c:10]:[c:11]:1-[C;D1;H3:12]>>[#16:6]-[#7;a:5]1:[c:4]:[c:3]:[c:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:7]1:[c:8]:[#16;a:9]:[c:10]:[c:11]:1-[C;D1;H3:12]
64.1
[{"value": 64.0, "product": "CN(C(OC(C)(C)C)=O)CC1=CN(C(=C1)C1=CSC=C1C)S(=O)(=O)C=1C=NC=CC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 64.1, "product": "CN(C(OC(C)(C)C)=O)CC1=CN(C(=C1)C1=CSC=C1C)S(=O)(=O)C=1C=NC=CC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
105
CELSIUS
18
HOUR
By a similar operation as in Reference Example 79 and using tert-butyl{[5-bromo-1-(pyridin-3-ylsulfonyl)-1H-pyrrol-3-yl]methyl}methylcarbamate (300 mg), (4-methyl-3-thienyl)boronic acid (198 mg), tetrakis(triphenylphosphine)palladium (40 mg) and sodium carbonate (222 mg), the title compound was obtained as a pale-yello...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1cc[nH]c1.c1ccsc1
c1ccsc1.c1cc[nH]c1
c1ccsc1.c1cc[nH]c1.c1ccncc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC
105
18
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.Cc1cscc1B(O)O>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC>Cc1cscc1-c1cc(CN(C)C(=O)OC(C)(C)C)cn1S(=O)(=O)c1cccnc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c773ef10de904febbe70cd25be98166e
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.N#Cc1cccc(B(O)O)c1>>CN(Cc1cc(-c2cccc(C#N)c2)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
C([O-])([O-])=O.[Na+].[Na+].C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)Br)S(=O)(=O)C=1C=NC=CC1)=O.C(#N)C=1C=C(C=CC1)B(O)O>>C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)C1=CC(=CC=C1)C#N)S(=O)(=O)C=1C=NC=CC1)=O
Br[c:6]1[cH:5][c:4]([CH2:3][N:2]([CH3:1])[C:26](=[O:27])[O:28][C:29]([CH3:30])([CH3:31])[CH3:32])[cH:25][n:15]1[S:16](=[O:17])(=[O:18])[c:19]1[cH:20][cH:21][cH:22][n:23][cH:24]1.OB(O)[c:7]1[cH:8][cH:9][cH:10][c:11]([C:12]#[N:13])[cH:14]1>>[CH3:1][N:2]([CH2:3][c:4]1[cH:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][c:11]([C:12]#[N:...
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.N#Cc1cccc(B(O)O)c1
CN(Cc1cc(-c2cccc(C#N)c2)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
null
C-C Coupling
Suzuki coupling with boronic acids
b71c1accb23fcf6e808cbf7fdd27a50d721fbf67e253875213e991e29cdecd2f
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[#7;a:5]:1-[#16:6].O-B(-O)-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10]:[c:11]>>[#16:6]-[#7;a:5]1:[c:4]:[c:3]:[c:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10]:[c:11]
94
[{"value": 94.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a similar operation as in Reference Example 79 and using tert-butyl{[5-bromo-1-(pyridin-3-ylsulfonyl)-1H-pyrrol-3-yl]methyl}methylcarbamate (300 mg), (3-cyanophenyl)boronic acid (205 mg), tetrakis(triphenylphosphine)palladium (40 mg) and sodium carbonate (222 mg), the title compound was obtained as a pale-yellow oil...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1cc[nH]c1.c1ccccc1
c1cc[nH]c1.c1ccccc1
c1cc[nH]c1.c1ccccc1.c1ccncc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
null
null
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.N#Cc1cccc(B(O)O)c1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1>CN(Cc1cc(-c2cccc(C#N)c2)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c291a2317c484540b4455ca73f844837
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.OB(O)c1ccccc1Cl>>CN(Cc1cc(-c2ccccc2Cl)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
C([O-])([O-])=O.[Na+].[Na+].C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)Br)S(=O)(=O)C=1C=NC=CC1)=O.ClC1=C(C=CC=C1)B(O)O>>C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)C1=C(C=CC=C1)Cl)S(=O)(=O)C=1C=NC=CC1)=O
Br[c:6]1[cH:5][c:4]([CH2:3][N:2]([CH3:1])[C:25](=[O:26])[O:27][C:28]([CH3:29])([CH3:30])[CH3:31])[cH:24][n:14]1[S:15](=[O:16])(=[O:17])[c:18]1[cH:19][cH:20][cH:21][n:22][cH:23]1.OB(O)[c:7]1[cH:8][cH:9][cH:10][cH:11][c:12]1[Cl:13]>>[CH3:1][N:2]([CH2:3][c:4]1[cH:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][cH:11][c:12]2[Cl:13])[n:...
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.OB(O)c1ccccc1Cl
CN(Cc1cc(-c2ccccc2Cl)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
null
C-C Coupling
Suzuki coupling with boronic acids
b71c1accb23fcf6e808cbf7fdd27a50d721fbf67e253875213e991e29cdecd2f
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[#7;a:5]:1-[#16:6].O-B(-O)-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10](-[Cl;D1;H0:11]):[c:12]>>[#16:6]-[#7;a:5]1:[c:4]:[c:3]:[c:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10](-[Cl;D1;H0:11]):[c:12]
53
[{"value": 53.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a similar operation as in Reference Example 79 and using tert-butyl{[5-bromo-1-(pyridin-3-ylsulfonyl)-1H-pyrrol-3-yl]methyl}methylcarbamate (300 mg), (2-chlorophenyl)boronic acid (218 mg), tetrakis(triphenylphosphine)palladium (40 mg) and sodium carbonate (222 mg), the title compound was obtained as a pale-blue oil ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1cc[nH]c1.c1ccccc1
c1cc[nH]c1.c1ccccc1
c1cc[nH]c1.c1ccccc1.c1ccncc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
null
null
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.OB(O)c1ccccc1Cl>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1>CN(Cc1cc(-c2ccccc2Cl)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-537e42143802433688494580d41cacc3
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.OB(O)c1ccc(F)cc1F>>CN(Cc1c[nH]c(-c2ccc(F)cc2F)c1)C(=O)OC(C)(C)C
C([O-])([O-])=O.[Na+].[Na+].C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)Br)S(=O)(=O)C=1C=NC=CC1)=O.FC1=C(C=CC(=C1)F)B(O)O>>C(C)(C)(C)OC(N(C)CC1=CNC(=C1)C1=C(C=C(C=C1)F)F)=O
O=S(=O)(c1cccnc1)[n:6]1[cH:5][c:4]([CH2:3][N:2]([CH3:1])[C:17](=[O:18])[O:19][C:20]([CH3:21])([CH3:22])[CH3:23])[cH:16][c:7]1Br.OB(O)[c:8]1[cH:9][cH:10][c:11]([F:12])[cH:13][c:14]1[F:15]>>[CH3:1][N:2]([CH2:3][c:4]1[cH:5][nH:6][c:7](-[c:8]2[cH:9][cH:10][c:11]([F:12])[cH:13][c:14]2[F:15])[cH:16]1)[C:17](=[O:18])[O:19][C:...
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.OB(O)c1ccc(F)cc1F
CN(Cc1c[nH]c(-c2ccc(F)cc2F)c1)C(=O)OC(C)(C)C
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
null
C-C Coupling
OtherReaction
091797deef34c648fc8f896a383f479af080cd2125994befadf3158dd8a13626
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc[nH]2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[n;H0;D3;+0:5]:1-S(=O)(=O)-c1:c:c:c:n:c:1.O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9](-[F;D1;H0:10]):[c:11]>>[F;D1;H0:10]-[c:9](:[c:11]):[c;H0;D3;+0:6](-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[nH;D2;+0:5]:1):[c:7]:[c:8]
50
[{"value": 50.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a similar operation as in Reference Example 79 and using tert-butyl{[5-bromo-1-(pyridin-3-ylsulfonyl)-1H-pyrrol-3-yl]methyl}methylcarbamate (300 mg), (2,4-difluorophenyl)boronic acid (198 mg), tetrakis(triphenylphosphine)palladium (40 mg) and sodium carbonate (220 mg), the title compound was obtained as a colorless ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccncc1.c1cc[nH]c1.c1ccccc1
c1cc[nH]c1.c1ccccc1
c1cc[nH]c1.c1ccccc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
null
null
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.OB(O)c1ccc(F)cc1F>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1>CN(Cc1c[nH]c(-c2ccc(F)cc2F)c1)C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-778b1e581a6d487490d6d5b28bd756f2
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.OB(O)c1cc(F)ccc1F>>CN(Cc1c[nH]c(-c2cc(F)ccc2F)c1)C(=O)OC(C)(C)C
C([O-])([O-])=O.[Na+].[Na+].C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)Br)S(=O)(=O)C=1C=NC=CC1)=O.FC1=C(C=C(C=C1)F)B(O)O>>C(C)(C)(C)OC(N(C)CC1=CNC(=C1)C1=C(C=CC(=C1)F)F)=O
O=S(=O)(c1cccnc1)[n:6]1[cH:5][c:4]([CH2:3][N:2]([CH3:1])[C:17](=[O:18])[O:19][C:20]([CH3:21])([CH3:22])[CH3:23])[cH:16][c:7]1Br.OB(O)[c:8]1[cH:9][c:10]([F:11])[cH:12][cH:13][c:14]1[F:15]>>[CH3:1][N:2]([CH2:3][c:4]1[cH:5][nH:6][c:7](-[c:8]2[cH:9][c:10]([F:11])[cH:12][cH:13][c:14]2[F:15])[cH:16]1)[C:17](=[O:18])[O:19][C:...
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.OB(O)c1cc(F)ccc1F
CN(Cc1c[nH]c(-c2cc(F)ccc2F)c1)C(=O)OC(C)(C)C
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
null
C-C Coupling
OtherReaction
091797deef34c648fc8f896a383f479af080cd2125994befadf3158dd8a13626
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc[nH]2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[n;H0;D3;+0:5]:1-S(=O)(=O)-c1:c:c:c:n:c:1.O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9](-[F;D1;H0:10]):[c:11]>>[F;D1;H0:10]-[c:9](:[c:11]):[c;H0;D3;+0:6](-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[nH;D2;+0:5]:1):[c:7]:[c:8]
60
[{"value": 60.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a similar operation as in Reference Example 79 and using tert-butyl{[5-bromo-1-(pyridin-3-ylsulfonyl)-1H-pyrrol-3-yl]methyl}methylcarbamate (300 mg), (2,5-difluorophenyl)boronic acid (220 mg), tetrakis(triphenylphosphine)palladium (40 mg) and sodium carbonate (220 mg), the title compound was obtained as a colorless ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccncc1.c1cc[nH]c1.c1ccccc1
c1cc[nH]c1.c1ccccc1
c1cc[nH]c1.c1ccccc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
null
null
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.OB(O)c1cc(F)ccc1F>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1>CN(Cc1c[nH]c(-c2cc(F)ccc2F)c1)C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c6dfb6ae20ff4eccbcd8f38bf24e4808
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.OB(O)c1ccc(Cl)cc1F>>CN(Cc1c[nH]c(-c2ccc(Cl)cc2F)c1)C(=O)OC(C)(C)C
C([O-])([O-])=O.[Na+].[Na+].C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)Br)S(=O)(=O)C=1C=NC=CC1)=O.ClC1=CC(=C(C=C1)B(O)O)F>>C(C)(C)(C)OC(N(C)CC1=CNC(=C1)C1=C(C=C(C=C1)Cl)F)=O
O=S(=O)(c1cccnc1)[n:6]1[cH:5][c:4]([CH2:3][N:2]([CH3:1])[C:17](=[O:18])[O:19][C:20]([CH3:21])([CH3:22])[CH3:23])[cH:16][c:7]1Br.OB(O)[c:8]1[cH:9][cH:10][c:11]([Cl:12])[cH:13][c:14]1[F:15]>>[CH3:1][N:2]([CH2:3][c:4]1[cH:5][nH:6][c:7](-[c:8]2[cH:9][cH:10][c:11]([Cl:12])[cH:13][c:14]2[F:15])[cH:16]1)[C:17](=[O:18])[O:19][...
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.OB(O)c1ccc(Cl)cc1F
CN(Cc1c[nH]c(-c2ccc(Cl)cc2F)c1)C(=O)OC(C)(C)C
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
null
C-C Coupling
OtherReaction
091797deef34c648fc8f896a383f479af080cd2125994befadf3158dd8a13626
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc[nH]2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[n;H0;D3;+0:5]:1-S(=O)(=O)-c1:c:c:c:n:c:1.O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9](-[F;D1;H0:10]):[c:11]>>[F;D1;H0:10]-[c:9](:[c:11]):[c;H0;D3;+0:6](-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[nH;D2;+0:5]:1):[c:7]:[c:8]
54
[{"value": 54.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a similar operation as in Reference Example 79 and using tert-butyl{[5-bromo-1-(pyridin-3-ylsulfonyl)-1H-pyrrol-3-yl]methyl}methylcarbamate (300 mg), (4-chloro-2-fluorophenyl)boronic acid (243 mg), tetrakis(triphenylphosphine)palladium (40 mg) and sodium carbonate (220 mg), the title compound was obtained as a color...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccncc1.c1cc[nH]c1.c1ccccc1
c1cc[nH]c1.c1ccccc1
c1cc[nH]c1.c1ccccc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
null
null
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.OB(O)c1ccc(Cl)cc1F>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1>CN(Cc1c[nH]c(-c2ccc(Cl)cc2F)c1)C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-25e31368fc4742eeab8df861801592a1
CN(Cc1c[nH]c(-c2ccc(F)cc2F)c1)C(=O)OC(C)(C)C.O=S(=O)(Cl)c1cccnc1>>CN(Cc1cc(-c2ccc(F)cc2F)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
C1COCCOCCOCCOCCO1.C(C)(C)(C)OC(N(C)CC1=CNC(=C1)C1=C(C=C(C=C1)F)F)=O.Cl.N1=CC(=CC=C1)S(=O)(=O)Cl.[H-].[Na+]>>C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)C1=C(C=C(C=C1)F)F)S(=O)(=O)C=1C=NC=CC1)=O
[CH3:1][N:2]([CH2:3][c:4]1[cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([F:11])[cH:12][c:13]2[F:14])[nH:15][cH:25]1)[C:26](=[O:27])[O:28][C:29]([CH3:30])([CH3:31])[CH3:32].Cl[S:16](=[O:17])(=[O:18])[c:19]1[cH:20][cH:21][cH:22][n:23][cH:24]1>>[CH3:1][N:2]([CH2:3][c:4]1[cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([F:11])[cH:12][c:13]2[...
CN(Cc1c[nH]c(-c2ccc(F)cc2F)c1)C(=O)OC(C)(C)C.O=S(=O)(Cl)c1cccnc1
CN(Cc1cc(-c2ccc(F)cc2F)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
null
null
null
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8].[c:9]-[c:10]1:[c:11]:[c:12]:[c:13]:[nH;D2;+0:14]:1>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8])-[n;H0;D3;+0:14]1:[c:13]:[c:12]:[c:11]:[c:10]:1-[c:9]
68
[{"value": 68.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a similar operation as in Reference Example 44 and using tert-butyl{[5-(2,4-difluorophenyl)-1H-pyrrol-3-yl]methyl}methylcarbamate (113 mg), sodium hydride (60% in oil, 51 mg), 15-crown-5 (0.21 mL) and pyridine-3-ylsulfonyl chloride hydrochloride (113 mg), the title compound was obtained as a pale-yellow oil (yield 1...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccccc1.c1ccncc1
HCl
null
null
null
CN(Cc1c[nH]c(-c2ccc(F)cc2F)c1)C(=O)OC(C)(C)C.O=S(=O)(Cl)c1cccnc1>>CN(Cc1cc(-c2ccc(F)cc2F)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-123e1f94be234b11acb7f52296716d61
CN(Cc1c[nH]c(-c2cc(F)ccc2F)c1)C(=O)OC(C)(C)C.O=S(=O)(Cl)c1cccnc1>>CN(Cc1cc(-c2cc(F)ccc2F)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
C1COCCOCCOCCOCCO1.C(C)(C)(C)OC(N(C)CC1=CNC(=C1)C1=C(C=CC(=C1)F)F)=O.Cl.N1=CC(=CC=C1)S(=O)(=O)Cl.[H-].[Na+]>>C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)C1=C(C=CC(=C1)F)F)S(=O)(=O)C=1C=NC=CC1)=O
[CH3:1][N:2]([CH2:3][c:4]1[cH:5][c:6](-[c:7]2[cH:8][c:9]([F:10])[cH:11][cH:12][c:13]2[F:14])[nH:15][cH:25]1)[C:26](=[O:27])[O:28][C:29]([CH3:30])([CH3:31])[CH3:32].Cl[S:16](=[O:17])(=[O:18])[c:19]1[cH:20][cH:21][cH:22][n:23][cH:24]1>>[CH3:1][N:2]([CH2:3][c:4]1[cH:5][c:6](-[c:7]2[cH:8][c:9]([F:10])[cH:11][cH:12][c:13]2[...
CN(Cc1c[nH]c(-c2cc(F)ccc2F)c1)C(=O)OC(C)(C)C.O=S(=O)(Cl)c1cccnc1
CN(Cc1cc(-c2cc(F)ccc2F)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
null
null
null
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8].[c:9]-[c:10]1:[c:11]:[c:12]:[c:13]:[nH;D2;+0:14]:1>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8])-[n;H0;D3;+0:14]1:[c:13]:[c:12]:[c:11]:[c:10]:1-[c:9]
54
[{"value": 54.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a similar operation as in Reference Example 44 and using tert-butyl{[5-(2,5-difluorophenyl)-1H-pyrrol-3-yl]methyl}methylcarbamate (135 mg), sodium hydride (60% in oil, 60 mg), 15-crown-5 (0.25 mL) and pyridin-3-ylsulfonyl chloride hydrochloride (135 mg), the title compound was obtained as a colorless oil (yield 105 ...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccccc1.c1ccncc1
HCl
null
null
null
CN(Cc1c[nH]c(-c2cc(F)ccc2F)c1)C(=O)OC(C)(C)C.O=S(=O)(Cl)c1cccnc1>>CN(Cc1cc(-c2cc(F)ccc2F)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3709138e248f4416a2c8559a917735b5
CN(Cc1c[nH]c(-c2ccc(Cl)cc2F)c1)C(=O)OC(C)(C)C.O=S(=O)(Cl)c1cccnc1>>CN(Cc1cc(-c2ccc(Cl)cc2F)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
C1COCCOCCOCCOCCO1.ClC1=CC(=C(C=C1)C1=CC(=CN1)CN(C(OC(C)(C)C)=O)C)F.Cl.N1=CC(=CC=C1)S(=O)(=O)Cl.[H-].[Na+]>>ClC1=CC(=C(C=C1)C1=CC(=CN1S(=O)(=O)C=1C=NC=CC1)CN(C(OC(C)(C)C)=O)C)F
[CH3:1][N:2]([CH2:3][c:4]1[cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([Cl:11])[cH:12][c:13]2[F:14])[nH:15][cH:25]1)[C:26](=[O:27])[O:28][C:29]([CH3:30])([CH3:31])[CH3:32].Cl[S:16](=[O:17])(=[O:18])[c:19]1[cH:20][cH:21][cH:22][n:23][cH:24]1>>[CH3:1][N:2]([CH2:3][c:4]1[cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([Cl:11])[cH:12][c:13]...
CN(Cc1c[nH]c(-c2ccc(Cl)cc2F)c1)C(=O)OC(C)(C)C.O=S(=O)(Cl)c1cccnc1
CN(Cc1cc(-c2ccc(Cl)cc2F)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
null
null
null
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8].[c:9]-[c:10]1:[c:11]:[c:12]:[c:13]:[nH;D2;+0:14]:1>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8])-[n;H0;D3;+0:14]1:[c:13]:[c:12]:[c:11]:[c:10]:1-[c:9]
57
[{"value": 57.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a similar operation as in Reference Example 44 and using tert-butyl {[5-(4-chloro-2-fluorophenyl)-1H-pyrrol-3-yl]methyl}methylcarbamate (127 mg), sodium hydride (60% in oil, 54 mg), 15-crown-5 (0.22 mL) and pyridin-3-ylsulfonyl chloride hydrochloride (120 mg), the title compound was obtained as a colorless oil (yiel...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccccc1.c1ccncc1
HCl
null
null
null
CN(Cc1c[nH]c(-c2ccc(Cl)cc2F)c1)C(=O)OC(C)(C)C.O=S(=O)(Cl)c1cccnc1>>CN(Cc1cc(-c2ccc(Cl)cc2F)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-96041b679b8d4334a31090cbd03cae3b
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.OB(O)c1cccc(F)c1>>CN(Cc1cc(-c2cccc(F)c2)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
C([O-])([O-])=O.[Na+].[Na+].C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)Br)S(=O)(=O)C=1C=NC=CC1)=O.FC=1C=C(C=CC1)B(O)O>>C(C)(C)(C)OC(N(C)CC1=CN(C(=C1)C1=CC(=CC=C1)F)S(=O)(=O)C=1C=NC=CC1)=O
Br[c:6]1[cH:5][c:4]([CH2:3][N:2]([CH3:1])[C:25](=[O:26])[O:27][C:28]([CH3:29])([CH3:30])[CH3:31])[cH:24][n:14]1[S:15](=[O:16])(=[O:17])[c:18]1[cH:19][cH:20][cH:21][n:22][cH:23]1.OB(O)[c:7]1[cH:8][cH:9][cH:10][c:11]([F:12])[cH:13]1>>[CH3:1][N:2]([CH2:3][c:4]1[cH:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][c:11]([F:12])[cH:13]2)[...
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.OB(O)c1cccc(F)c1
CN(Cc1cc(-c2cccc(F)c2)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
null
C-C Coupling
Suzuki coupling with boronic acids
b71c1accb23fcf6e808cbf7fdd27a50d721fbf67e253875213e991e29cdecd2f
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[#7;a:5]:1-[#16:6].O-B(-O)-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10]:[c:11]>>[#16:6]-[#7;a:5]1:[c:4]:[c:3]:[c:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10]:[c:11]
90
[{"value": 90.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a similar operation as in Reference Example 79 and using tert-butyl{[5-bromo-1-(pyridin-3-ylsulfonyl)-1H-pyrrol-3-yl]methyl}methylcarbamate (300 mg), (3-fluorophenyl)boronic acid (195 mg), tetrakis(triphenylphosphine)palladium (40 mg) and sodium carbonate (222 mg), the title compound was obtained as a pale-yellow oi...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1cc[nH]c1.c1ccccc1
c1cc[nH]c1.c1ccccc1
c1cc[nH]c1.c1ccccc1.c1ccncc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
null
null
CN(Cc1cc(Br)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C.OB(O)c1cccc(F)c1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1>CN(Cc1cc(-c2cccc(F)c2)n(S(=O)(=O)c2cccnc2)c1)C(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a333f877b8bd4db78a5049562ef794dd
BrBr.CC(=O)c1c(F)cccc1F>>O=C(CBr)c1c(F)cccc1F
O.BrBr.FC1=C(C(=CC=C1)F)C(C)=O.[Cl-].[Al+3].[Cl-].[Cl-]>>BrCC(=O)C1=C(C=CC=C1F)F
Br[Br:4].[O:1]=[C:2]([CH3:3])[c:5]1[c:6]([F:7])[cH:8][cH:9][cH:10][c:11]1[F:12]>>[O:1]=[C:2]([CH2:3][Br:4])[c:5]1[c:6]([F:7])[cH:8][cH:9][cH:10][c:11]1[F:12]
BrBr.CC(=O)c1c(F)cccc1F
O=C(CBr)c1c(F)cccc1F
null
null
C(C)OCC
Functional Group Interconversion
Bromination
97ca6720945af5a02c450d33ec56e946521050f9771c27f9cfcb85f3477593f6
cb3e14519230141aa015a4cf9c960def3e60f01997e61621f62506924bfa15de
c1ccccc1
Br-[Br;H0;D1;+0:1].[CH3;D1;+0:2]-[C:3](=[O;D1;H0:4])-[c:5]>>[Br;H0;D1;+0:1]-[CH2;D2;+0:2]-[C:3](=[O;D1;H0:4])-[c:5]
100
[{"value": 100.0, "product": "BrCC(=O)C1=C(C=CC=C1F)F", "details": "PERCENTYIELD", "is_desired": false}]
null
null
5
MINUTE
To a solution of 1-(2,6-difluorophenyl)ethanone (10.0 g) in diethyl ether (50 mL) was added anhydrous aluminum chloride (86 mg) and the mixture was stirred for 5 min. Bromine (3.3 mL) was added dropwise at 10-15° C. After stirring at room temperature for 2 hr, the mixture was poured into water, and the mixture was extr...
10.6084/m9.figshare.5104873.v1
null
Ketone
Primary halide
null
null
c1ccccc1
HBr
C(C)OCC
null
0.083333
BrBr.CC(=O)c1c(F)cccc1F>C(C)OCC>O=C(CBr)c1c(F)cccc1F
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-105a8ca46e104d9084d71d0ffe892f07
CCOC(=O)CC#N.O=C(CBr)c1c(F)cccc1F>>CCOC(=O)C(C#N)CC(=O)c1c(F)cccc1F
C(#N)CC(=O)OCC.C(C)(C)N(CC)C(C)C.BrCC(=O)C1=C(C=CC=C1F)F>>C(#N)C(C(=O)OCC)CC(=O)C1=C(C=CC=C1F)F
[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][C:7]#[N:8].Br[CH2:9][C:10](=[O:11])[c:12]1[c:13]([F:14])[cH:15][cH:16][cH:17][c:18]1[F:19]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]([C:7]#[N:8])[CH2:9][C:10](=[O:11])[c:12]1[c:13]([F:14])[cH:15][cH:16][cH:17][c:18]1[F:19]
CCOC(=O)CC#N.O=C(CBr)c1c(F)cccc1F
CCOC(=O)C(C#N)CC(=O)c1c(F)cccc1F
null
null
O1CCCC1
C-C Coupling
OtherReaction
8f6d4b304f760571a184e9fdd40a1eea1ac2caef68076ef062be84edd531cf09
4c05eab7fc11daae7c29afd57dcd00ee6caafc643a857cb0c2660dc4a28e52eb
c1ccccc1
Br-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4].[C:5]-[#8:6]-[C:7](=[O;D1;H0:8])-[CH2;D2;+0:9]-[C:10]#[N;D1;H0:11]>>[C:5]-[#8:6]-[C:7](=[O;D1;H0:8])-[CH;D3;+0:9](-[C:10]#[N;D1;H0:11])-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]
81
[{"value": 81.0, "product": "C(#N)C(C(=O)OCC)CC(=O)C1=C(C=CC=C1F)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 80.7, "product": "C(#N)C(C(=O)OCC)CC(=O)C1=C(C=CC=C1F)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
12
HOUR
To a solution of ethyl cyanoacetate (7.24 g) and diisopropylethylamine (19.9 g) in tetrahydrofuran (30 mL) was added dropwise a solution of 2-bromo-1-(2,6-difluorophenyl)ethanone (15.16 g) in tetrahydrofuran (15 mL) at 10-15° C. The mixture was stirred at room temperature for 12 hr. The reaction mixture was filtered, a...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ketone.Ester
Ketone.Ester
null
null
c1ccccc1
HBr
O1CCCC1
null
12
CCOC(=O)CC#N.O=C(CBr)c1c(F)cccc1F>O1CCCC1>CCOC(=O)C(C#N)CC(=O)c1c(F)cccc1F
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d84b5e71971e4e41b5b48b9f3f750528
CCOC(=O)C(C#N)CC(=O)c1c(F)cccc1F.Cl>>CCOC(=O)c1cc(-c2c(F)cccc2F)[nH]c1Cl
C(#N)C(C(=O)OCC)CC(=O)C1=C(C=CC=C1F)F.C(C)(=O)OCC.Cl>>ClC=1NC(=CC1C(=O)OCC)C1=C(C=CC=C1F)F
O=[C:8]([CH2:7][CH:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[C:18]#[N:17])[c:9]1[c:10]([F:11])[cH:12][cH:13][cH:14][c:15]1[F:16].[ClH:19]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][c:8](-[c:9]2[c:10]([F:11])[cH:12][cH:13][cH:14][c:15]2[F:16])[nH:17][c:18]1[Cl:19]
CCOC(=O)C(C#N)CC(=O)c1c(F)cccc1F.Cl
CCOC(=O)c1cc(-c2c(F)cccc2F)[nH]c1Cl
null
null
C(C)(=O)OCC
Aromatic Heterocycle Formation
OtherReaction
ee999686a7991e07d7c287a446be67936cb0259cc7da34bde8489e32aa619966
463beee1c06ff6990c2e1332d51dae761cf1d15bf3cb1e31ff2630a30ad5b435
c1ccc(-c2ccc[nH]2)cc1
O=[C;H0;D3;+0:1](-[CH2;D2;+0:2]-[CH;D3;+0:3](-[C;H0;D2;+0:4]#[N;H0;D1;+0:5])-[C:6](=[O;D1;H0:7])-[#8:8]-[C:9])-[c;H0;D3;+0:10](:[c:11](-[F;D1;H0:12]):[c:13]):[c:14](-[F;D1;H0:15]):[c:16].[ClH;D0;+0:17]>>[C:9]-[#8:8]-[C:6](=[O;D1;H0:7])-[c;H0;D3;+0:3]1:[cH;D2;+0:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:10](:[c:11](-[F;D1;H0:12]):...
68
[{"value": 68.0, "product": "ClC=1NC(=CC1C(=O)OCC)C1=C(C=CC=C1F)F", "details": "PERCENTYIELD", "is_desired": false}]
null
null
12
HOUR
A solution (14 mL) of ethyl 2-cyano-4-(2,6-difluorophenyl)-4-oxobutanoate (13.83 g) in ethyl acetate was added dropwise to 4 mol/L hydrogen chloride-ethyl acetate solution (100 mL) at 10-15° C. The mixture was stirred at room temperature for 12 hr, and concentrated under reduced pressure. The residue was purified by si...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ester.Nitrile
Aromatic halide.Ester
null
c1cc[nH]c1
c1cc[nH]c1.c1ccccc1
HO-
C(C)(=O)OCC
null
12
CCOC(=O)C(C#N)CC(=O)c1c(F)cccc1F.Cl>C(C)(=O)OCC>CCOC(=O)c1cc(-c2c(F)cccc2F)[nH]c1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9bde0efe4776456b93ee9a0bc799c1cb
COC(=O)C(C#N)CC(=O)c1ccc(C2CCCCC2)cc1.Cl>>COC(=O)c1cc(-c2ccc(C3CCCCC3)cc2)[nH]c1Cl
C(#N)C(C(=O)OC)CC(=O)C1=CC=C(C=C1)C1CCCCC1.O1CCOCC1.Cl>>ClC=1NC(=CC1C(=O)OC)C1=CC=C(C=C1)C1CCCCC1
O=[C:7]([CH2:6][CH:5]([C:3]([O:2][CH3:1])=[O:4])[C:21]#[N:20])[c:8]1[cH:9][cH:10][c:11]([CH:12]2[CH2:13][CH2:14][CH2:15][CH2:16][CH2:17]2)[cH:18][cH:19]1.[ClH:22]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7](-[c:8]2[cH:9][cH:10][c:11]([CH:12]3[CH2:13][CH2:14][CH2:15][CH2:16][CH2:17]3)[cH:18][cH:19]2)[nH:20][c:21]1[Cl:22...
COC(=O)C(C#N)CC(=O)c1ccc(C2CCCCC2)cc1.Cl
COC(=O)c1cc(-c2ccc(C3CCCCC3)cc2)[nH]c1Cl
null
null
null
Aromatic Heterocycle Formation
OtherReaction
ee999686a7991e07d7c287a446be67936cb0259cc7da34bde8489e32aa619966
463beee1c06ff6990c2e1332d51dae761cf1d15bf3cb1e31ff2630a30ad5b435
c1c[nH]c(-c2ccc(C3CCCCC3)cc2)c1
O=[C;H0;D3;+0:1](-[CH2;D2;+0:2]-[CH;D3;+0:3](-[C;H0;D2;+0:4]#[N;H0;D1;+0:5])-[C:6](=[O;D1;H0:7])-[#8:8]-[C;D1;H3:9])-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14].[ClH;D0;+0:15]>>[C;D1;H3:9]-[#8:8]-[C:6](=[O;D1;H0:7])-[c;H0;D3;+0:3]1:[cH;D2;+0:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]):[nH;D2;+0:...
null
[]
null
null
8
HOUR
14% Hydrogen chloride-1,4-dioxane solution (50 mL) was added to methyl 2-cyano-4-(4-cyclohexylphenyl)-4-oxobutanoate (12.1 g) and the mixture was stirred at room temperature for 8 hr and concentrated under reduced pressure. The residue was dissolved in ethyl acetate, washed with saturated brine, dried over anhydrous ma...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ester.Nitrile
Aromatic halide.Ester
null
c1cc[nH]c1
c1cc[nH]c1.c1ccccc1.C1CCCCC1
HO-
null
null
8
COC(=O)C(C#N)CC(=O)c1ccc(C2CCCCC2)cc1.Cl>>COC(=O)c1cc(-c2ccc(C3CCCCC3)cc2)[nH]c1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-519ff4b97d5e4f4da47a7cf86aa0eda5
COC(=O)c1cc(-c2ccccc2)[nH]c1Cl>>COC(=O)c1c(Cl)[nH]c(-c2ccccc2)c1F
C(#N)CC(=O)OC.C(C(=O)C1=CC=CC=C1)Br.[O-]S(=O)(=O)C(F)(F)F.ClC1=[N+](C(=CC=C1)Cl)F.ClC=1NC(=CC1C(=O)OC)C1=CC=CC=C1>>ClC=1NC(=C(C1C(=O)OC)F)C1=CC=CC=C1
[CH3:1][O:2][C:3](=[O:4])[c:5]1[c:6]([Cl:7])[nH:8][c:9](-[c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[cH:16]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[c:6]([Cl:7])[nH:8][c:9](-[c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[c:16]1[F:17]
COC(=O)c1cc(-c2ccccc2)[nH]c1Cl
COC(=O)c1c(Cl)[nH]c(-c2ccccc2)c1F
null
null
C(C)#N
Functional Group Addition
Aromatic fluorination
4048bac0b4c21eb6e694a585c03c487c6380befb41bf01d9388a95029c960e33
0a2f22058f27970cef4a98a778644dbe9c44e91f66c74cd24db321993177608a
c1ccc(-c2ccc[nH]2)cc1
[C;D1;H3:1]-[#8:2]-[C:3](=[O;D1;H0:4])-[c:5]1:[cH;D2;+0:6]:[c:7](-[c:8]):[#7;a:9]:[c:10]:1-[Cl;D1;H0:11]>>[C;D1;H3:1]-[#8:2]-[C:3](=[O;D1;H0:4])-[c:5]1:[c:10](-[Cl;D1;H0:11]):[#7;a:9]:[c:7](-[c:8]):[c;H0;D3;+0:6]:1-[F;D1;H0:12]
16.2
[{"value": 16.0, "product": "ClC=1NC(=C(C1C(=O)OC)F)C1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 16.2, "product": "ClC=1NC(=C(C1C(=O)OC)F)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
To a suspension of methyl 2-chloro-5-phenyl-1H-pyrrole-3-carboxylate (4.66 g) synthesized from methyl cyanoacetate and phenacyl bromide in the same manner as in Reference Example 95 and Reference Example 97 in acetonitrile (200 mL) was added 2,6-dichloro-N-fluoropyridinium triflate (6.26 g) over 10 min under ice-coolin...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccccc1
Other
C(C)#N
null
2
COC(=O)c1cc(-c2ccccc2)[nH]c1Cl>C(C)#N>COC(=O)c1c(Cl)[nH]c(-c2ccccc2)c1F
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9131238d8acb4969be2a977c7e6f285c
COC(=O)CC#N.O=C(CBr)c1ccccc1>>COC(=O)C(C#N)CC(=O)c1ccccc1
C(#N)CC(=O)OC.C(C)(C)N(CC)C(C)C.C(C(=O)C1=CC=CC=C1)Br>>C(#N)C(C(=O)OC)CC(=O)C1=CC=CC=C1
[CH3:1][O:2][C:3](=[O:4])[CH2:5][C:6]#[N:7].Br[CH2:8][C:9](=[O:10])[c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1>>[CH3:1][O:2][C:3](=[O:4])[CH:5]([C:6]#[N:7])[CH2:8][C:9](=[O:10])[c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1
COC(=O)CC#N.O=C(CBr)c1ccccc1
COC(=O)C(C#N)CC(=O)c1ccccc1
null
null
O1CCCC1
C-C Coupling
OtherReaction
8f6d4b304f760571a184e9fdd40a1eea1ac2caef68076ef062be84edd531cf09
4c05eab7fc11daae7c29afd57dcd00ee6caafc643a857cb0c2660dc4a28e52eb
c1ccccc1
Br-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4].[C;D1;H3:5]-[#8:6]-[C:7](=[O;D1;H0:8])-[CH2;D2;+0:9]-[C:10]#[N;D1;H0:11]>>[C;D1;H3:5]-[#8:6]-[C:7](=[O;D1;H0:8])-[CH;D3;+0:9](-[C:10]#[N;D1;H0:11])-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]
95
[{"value": 95.0, "product": "C(#N)C(C(=O)OC)CC(=O)C1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 94.6, "product": "C(#N)C(C(=O)OC)CC(=O)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
12
HOUR
To a suspension of methyl 2-chloro-5-phenyl-1H-pyrrole-3-carboxylate (4.66 g) synthesized from methyl cyanoacetate and phenacyl bromide in the same manner as in Reference Example 95 and Reference Example 97 in acetonitrile (200 mL) was added 2,6-dichloro-N-fluoropyridinium triflate (6.26 g) over 10 min under ice-coolin...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ketone.Ester
Ketone.Ester
null
null
c1ccccc1
HBr
O1CCCC1
null
12
COC(=O)CC#N.O=C(CBr)c1ccccc1>O1CCCC1>COC(=O)C(C#N)CC(=O)c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-de13114bf9624623a4cbd95d7e9ba88d
CCOC(=O)C(C#N)CC(=O)c1c(F)cccc1F.Cl>>COC(=O)c1cc(-c2ccccc2)[nH]c1Cl
C(#N)C(C(=O)OCC)CC(=O)C1=C(C=CC=C1F)F.C(C)(=O)OCC.Cl>>ClC=1NC(=CC1C(=O)OC)C1=CC=CC=C1
C[CH2:1][O:2][C:3](=[O:4])[CH:5]([CH2:6][C:7](=O)[c:8]1[c:9](F)[cH:10][cH:11][cH:12][c:13]1F)[C:15]#[N:14].[ClH:16]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7](-[c:8]2[cH:9][cH:10][cH:11][cH:12][cH:13]2)[nH:14][c:15]1[Cl:16]
CCOC(=O)C(C#N)CC(=O)c1c(F)cccc1F.Cl
COC(=O)c1cc(-c2ccccc2)[nH]c1Cl
null
null
C(C)(=O)OCC
Aromatic Heterocycle Formation
OtherReaction
35af3be39562adfa2ad324fe1de13666dad61852fa02459b726524c79d2f63a3
e7bd1d55a47c3e143d871399746cf3601c5840f5b888f86bbeb382863a5d68d7
c1ccc(-c2ccc[nH]2)cc1
C-[CH2;D2;+0:1]-[#8:2]-[C:3](=[O;D1;H0:4])-[CH;D3;+0:5](-[C;H0;D2;+0:6]#[N;H0;D1;+0:7])-[CH2;D2;+0:8]-[C;H0;D3;+0:9](=O)-[c;H0;D3;+0:10]1:[c;H0;D3;+0:11](-F):[c:12]:[c:13]:[c:14]:[c;H0;D3;+0:15]:1-F.[ClH;D0;+0:16]>>[CH3;D1;+0:1]-[#8:2]-[C:3](=[O;D1;H0:4])-[c;H0;D3;+0:5]1:[cH;D2;+0:8]:[c;H0;D3;+0:9](-[c;H0;D3;+0:10]2:[c...
37
[{"value": 37.0, "product": "ClC=1NC(=CC1C(=O)OC)C1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
18
HOUR
To a suspension of methyl 2-chloro-5-phenyl-1H-pyrrole-3-carboxylate (4.66 g) synthesized from methyl cyanoacetate and phenacyl bromide in the same manner as in Reference Example 95 and Reference Example 97 in acetonitrile (200 mL) was added 2,6-dichloro-N-fluoropyridinium triflate (6.26 g) over 10 min under ice-coolin...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide.Ketone.Ester.Nitrile
Aromatic halide.Ester
c1ccccc1
c1cc[nH]c1.c1ccccc1
c1cc[nH]c1.c1ccccc1
HF
C(C)(=O)OCC
null
18
CCOC(=O)C(C#N)CC(=O)c1c(F)cccc1F.Cl>C(C)(=O)OCC>COC(=O)c1cc(-c2ccccc2)[nH]c1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-220ec73cbe7346479395b32bd15ef6e2
CCOC(=O)c1cc(-c2c(F)cccc2F)[nH]c1Cl>>CCOC(=O)c1c[nH]c(-c2c(F)cccc2F)c1
ClC=1NC(=CC1C(=O)OCC)C1=C(C=CC=C1F)F>>FC1=C(C(=CC=C1)F)C1=CC(=CN1)C(=O)OCC
Cl[c:7]1[c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[cH:18][c:9](-[c:10]2[c:11]([F:12])[cH:13][cH:14][cH:15][c:16]2[F:17])[nH:8]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][nH:8][c:9](-[c:10]2[c:11]([F:12])[cH:13][cH:14][cH:15][c:16]2[F:17])[cH:18]1
CCOC(=O)c1cc(-c2c(F)cccc2F)[nH]c1Cl
CCOC(=O)c1c[nH]c(-c2c(F)cccc2F)c1
null
[C].[Pd]
C(C)O
Functional Group Interconversion
Aromatic dehalogenation
0ec084506a1195e403239281a55b47251adfd459417d17893b063b33c6f08040
56de34d4a44cb25d9380269ee5e138b0f24b40a3a0db22c5508049dc775a861f
c1ccc(-c2ccc[nH]2)cc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[#8:8]-[C:9]>>[C:9]-[#8:8]-[C:6](=[O;D1;H0:7])-[c:5]1:[c:4]:[c:3]:[#7;a:2]:[cH;D2;+0:1]:1
44
[{"value": 24.0, "product": "FC1=C(C(=CC=C1)F)C1=CC(=CN1)C(=O)OCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 44.0, "product": "FC1=C(C(=CC=C1)F)C1=CC(=CN1)C(=O)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
40
CELSIUS
72
HOUR
To a solution of ethyl 2-chloro-5-(2,6-difluorophenyl)-1H-pyrrole-3-carboxylate (9.82 g) in ethanol (200 mL) was added 10% palladium carbon (50% containing water, 4.91 g), and the mixture was stirred under a hydrogen atmosphere at 40° C. for 72 hr. The reaction mixture was filtered, and the filtrate was concentrated un...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccccc1
Other
[C].[Pd].C(C)O
40
72
CCOC(=O)c1cc(-c2c(F)cccc2F)[nH]c1Cl>[C].[Pd].C(C)O>CCOC(=O)c1c[nH]c(-c2c(F)cccc2F)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f8d5160f7d2d428798d929bface03fd7
COC(=O)c1cc(-c2ccc(C3CCCCC3)cc2)[nH]c1Cl>>COC(=O)c1c[nH]c(-c2ccc(C3CCCCC3)cc2)c1
ClC=1NC(=CC1C(=O)OC)C1=CC=C(C=C1)C1CCCCC1.NC=1OC(=CC1C(=O)OC)C1=CC=C(C=C1)C1CCCCC1>>C1(CCCCC1)C1=CC=C(C=C1)C1=CC(=CN1)C(=O)OC
Cl[c:6]1[c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:21][c:8](-[c:9]2[cH:10][cH:11][c:12]([CH:13]3[CH2:14][CH2:15][CH2:16][CH2:17][CH2:18]3)[cH:19][cH:20]2)[nH:7]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][nH:7][c:8](-[c:9]2[cH:10][cH:11][c:12]([CH:13]3[CH2:14][CH2:15][CH2:16][CH2:17][CH2:18]3)[cH:19][cH:20]2)[cH:21]1
COC(=O)c1cc(-c2ccc(C3CCCCC3)cc2)[nH]c1Cl
COC(=O)c1c[nH]c(-c2ccc(C3CCCCC3)cc2)c1
null
[C].[Pd]
CO.C(C)(=O)OCC
Functional Group Interconversion
Aromatic dehalogenation
0ec084506a1195e403239281a55b47251adfd459417d17893b063b33c6f08040
56de34d4a44cb25d9380269ee5e138b0f24b40a3a0db22c5508049dc775a861f
c1c[nH]c(-c2ccc(C3CCCCC3)cc2)c1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[#8:8]-[C;D1;H3:9]>>[C;D1;H3:9]-[#8:8]-[C:6](=[O;D1;H0:7])-[c:5]1:[c:4]:[c:3]:[#7;a:2]:[cH;D2;+0:1]:1
41.1
[{"value": 41.0, "product": "C1(CCCCC1)C1=CC=C(C=C1)C1=CC(=CN1)C(=O)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 41.1, "product": "C1(CCCCC1)C1=CC=C(C=C1)C1=CC(=CN1)C(=O)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
50
CELSIUS
14
HOUR
To a solution of a nearly 1:1 mixture (3.41 g) of methyl 2-chloro-5-(4-cyclohexylphenyl)-1H-pyrrole-3-carboxylate and methyl 2-amino-5-(4-cyclohexylphenyl)-3-furoate in methanol (30 mL) and ethyl acetate (10 mL) was added 10% palladium carbon (50% containing water, 0.34 g), and the mixture was stirred under a hydrogen ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccccc1.C1CCCCC1
Other
[C].[Pd].CO.C(C)(=O)OCC
50
14
COC(=O)c1cc(-c2ccc(C3CCCCC3)cc2)[nH]c1Cl>[C].[Pd].CO.C(C)(=O)OCC>COC(=O)c1c[nH]c(-c2ccc(C3CCCCC3)cc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d1d1310ec7044f80b7e27927a463a9dd
COC(=O)c1c(Cl)[nH]c(-c2ccccc2)c1F>>COC(=O)c1c[nH]c(-c2ccccc2)c1F
ClC=1NC(=C(C1C(=O)OC)F)C1=CC=CC=C1.C(C)N(CC)CC>>FC=1C(=CNC1C1=CC=CC=C1)C(=O)OC
Cl[c:6]1[c:5]([C:3]([O:2][CH3:1])=[O:4])[c:15]([F:16])[c:8](-[c:9]2[cH:10][cH:11][cH:12][cH:13][cH:14]2)[nH:7]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][nH:7][c:8](-[c:9]2[cH:10][cH:11][cH:12][cH:13][cH:14]2)[c:15]1[F:16]
COC(=O)c1c(Cl)[nH]c(-c2ccccc2)c1F
COC(=O)c1c[nH]c(-c2ccccc2)c1F
null
[C].[Pd]
CO
Functional Group Interconversion
Aromatic dehalogenation
0ec084506a1195e403239281a55b47251adfd459417d17893b063b33c6f08040
56de34d4a44cb25d9380269ee5e138b0f24b40a3a0db22c5508049dc775a861f
c1ccc(-c2ccc[nH]2)cc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[#8:8]-[C;D1;H3:9]>>[C;D1;H3:9]-[#8:8]-[C:6](=[O;D1;H0:7])-[c:5]1:[c:4]:[c:3]:[#7;a:2]:[cH;D2;+0:1]:1
86,784.9
[{"value": 87.0, "product": "FC=1C(=CNC1C1=CC=CC=C1)C(=O)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 86784.9, "product": "FC=1C(=CNC1C1=CC=CC=C1)C(=O)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
Methyl 2-chloro-4-fluoro-5-phenyl-1H-pyrrole-3-carboxylate (0.92 mg), 10% palladium carbon (50% containing water, 0.20 g) and triethylamine (0.56 mL) were suspended in methanol (30 mL), and the mixture was stirred under a hydrogen atmosphere at room temperature for 2 hr. The reaction mixture was filtered through celite...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccccc1
Other
[C].[Pd].CO
null
2
COC(=O)c1c(Cl)[nH]c(-c2ccccc2)c1F>[C].[Pd].CO>COC(=O)c1c[nH]c(-c2ccccc2)c1F
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b7ea2b2ed80244d19dc07e792bbb284a
CCOC(=O)c1c[nH]c(-c2c(F)cccc2F)c1>>OCc1c[nH]c(-c2c(F)cccc2F)c1
O.[H-].C(C(C)C)[Al+]CC(C)C.FC1=C(C(=CC=C1)F)C1=CC(=CN1)C(=O)OCC>>FC1=C(C(=CC=C1)F)C1=CC(=CN1)CO
CCO[C:2](=[O:1])[c:3]1[cH:4][nH:5][c:6](-[c:7]2[c:8]([F:9])[cH:10][cH:11][cH:12][c:13]2[F:14])[cH:15]1>>[OH:1][CH2:2][c:3]1[cH:4][nH:5][c:6](-[c:7]2[c:8]([F:9])[cH:10][cH:11][cH:12][c:13]2[F:14])[cH:15]1
CCOC(=O)c1c[nH]c(-c2c(F)cccc2F)c1
OCc1c[nH]c(-c2c(F)cccc2F)c1
null
null
O1CCCC1.C1(=CC=CC=C1)C.C(C)(=O)OCC.S(=O)(=O)([O-])[O-].[Mg+2]
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
c1ccc(-c2ccc[nH]2)cc1
C-C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[c:7]:1>>[OH;D1;+0:2]-[CH2;D2;+0:1]-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[c:7]:1
97
[{"value": 97.0, "product": "FC1=C(C(=CC=C1)F)C1=CC(=CN1)CO", "details": "PERCENTYIELD", "is_desired": false}, {"value": 96.8, "product": "FC1=C(C(=CC=C1)F)C1=CC(=CN1)CO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
A solution (35 mL) of ethyl 5-(2,6-difluorophenyl)-1H-pyrrole-3-carboxylate (3.35 g) in tetrahydrofuran was cooled to −50° C., and a 1.5 mol/L solution (30 mL) of diisobutylaluminum hydride in toluene was added dropwise by small portions. The mixture was stirred at the same temperature for 1 hr, water was added to the ...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
c1cc[nH]c1.c1ccccc1
HO-
O1CCCC1.C1(=CC=CC=C1)C.C(C)(=O)OCC.S(=O)(=O)([O-])[O-].[Mg+2]
null
1
CCOC(=O)c1c[nH]c(-c2c(F)cccc2F)c1>O1CCCC1.C1(=CC=CC=C1)C.C(C)(=O)OCC.S(=O)(=O)([O-])[O-].[Mg+2]>OCc1c[nH]c(-c2c(F)cccc2F)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ec06b0df98f54598b2ba320b02085040
COC(=O)c1c[nH]c(-c2ccc(C3CCCCC3)cc2)c1>>OCc1c[nH]c(-c2ccc(C3CCCCC3)cc2)c1
Cl.C1(CCCCC1)C1=CC=C(C=C1)C1=CC(=CN1)C(=O)OC.[H-].C(C(C)C)[Al+]CC(C)C>>C1(CCCCC1)C1=CC=C(C=C1)C1=CC(=CN1)CO
CO[C:2](=[O:1])[c:3]1[cH:4][nH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([CH:11]3[CH2:12][CH2:13][CH2:14][CH2:15][CH2:16]3)[cH:17][cH:18]2)[cH:19]1>>[OH:1][CH2:2][c:3]1[cH:4][nH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([CH:11]3[CH2:12][CH2:13][CH2:14][CH2:15][CH2:16]3)[cH:17][cH:18]2)[cH:19]1
COC(=O)c1c[nH]c(-c2ccc(C3CCCCC3)cc2)c1
OCc1c[nH]c(-c2ccc(C3CCCCC3)cc2)c1
null
null
O1CCCC1.C1(=CC=CC=C1)C.C(C)(=O)OCC
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
c1c[nH]c(-c2ccc(C3CCCCC3)cc2)c1
C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[c:7]:1>>[OH;D1;+0:2]-[CH2;D2;+0:1]-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[c:7]:1
40
[{"value": 40.0, "product": "C1(CCCCC1)C1=CC=C(C=C1)C1=CC(=CN1)CO", "details": "PERCENTYIELD", "is_desired": false}, {"value": 39.6, "product": "C1(CCCCC1)C1=CC=C(C=C1)C1=CC(=CN1)CO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
To a solution of methyl 5-(4-cyclohexylphenyl)-1H-pyrrole-3-carboxylate (3.0 g) in absolute tetrahydrofuran (40 mL) was added dropwise a 1.5 mol/L solution (21.0 mL) of diisobutylaluminum hydride in toluene at −78° C. The mixture was further stirred at the same temperature for 2 hr. To the reaction mixture was added 1 ...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
c1cc[nH]c1.c1ccccc1.C1CCCCC1
Other
O1CCCC1.C1(=CC=CC=C1)C.C(C)(=O)OCC
null
2
COC(=O)c1c[nH]c(-c2ccc(C3CCCCC3)cc2)c1>O1CCCC1.C1(=CC=CC=C1)C.C(C)(=O)OCC>OCc1c[nH]c(-c2ccc(C3CCCCC3)cc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6978548cbfd141b799db12b575d852a6
OCc1c[nH]c(-c2c(F)cccc2F)c1>>O=Cc1c[nH]c(-c2c(F)cccc2F)c1
FC1=C(C(=CC=C1)F)C1=CC(=CN1)CO.C[N+]1(CCOCC1)[O-]>>FC1=C(C(=CC=C1)F)C1=CC(=CN1)C=O
[OH:1][CH2:2][c:3]1[cH:4][nH:5][c:6](-[c:7]2[c:8]([F:9])[cH:10][cH:11][cH:12][c:13]2[F:14])[cH:15]1>>[O:1]=[CH:2][c:3]1[cH:4][nH:5][c:6](-[c:7]2[c:8]([F:9])[cH:10][cH:11][cH:12][c:13]2[F:14])[cH:15]1
OCc1c[nH]c(-c2c(F)cccc2F)c1
O=Cc1c[nH]c(-c2c(F)cccc2F)c1
null
[Ru](=O)(=O)(=O)[O-].C(CC)[N+](CCC)(CCC)CCC
C(C)#N.C(C)(=O)OCC
Oxidation
Oxidation or Dehydrogenation of Alcohols to Aldehydes and Ketones
41bfa9deea81b465c88ad21fdfb64a2e1ba29490558cf430df132cb98b4a538b
0a03c6724c1862e8f86d4a463afda55b8e067dc6cb42597b472eb7cabc03eda3
c1ccc(-c2ccc[nH]2)cc1
[OH;D1;+0:1]-[CH2;D2;+0:2]-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[c:7]:1>>[O;H0;D1;+0:1]=[CH;D2;+0:2]-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[c:7]:1
77
[{"value": 77.0, "product": "FC1=C(C(=CC=C1)F)C1=CC(=CN1)C=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 76.5, "product": "FC1=C(C(=CC=C1)F)C1=CC(=CN1)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
To a solution (26 mL) of [5-(2,6-difluorophenyl)-1H-pyrrol-3-yl]methanol (2.56 g) in acetonitrile were added tetra-n-propylammonium perruthenate (430 mg), N-methylmorpholine N-oxide (2.15 g) and molecular sieves 4A powder (5 g), and the mixture was stirred at room temperature for 2 hr. The reaction mixture was diluted ...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Aldehyde
null
null
c1cc[nH]c1.c1ccccc1
null
[Ru](=O)(=O)(=O)[O-].C(CC)[N+](CCC)(CCC)CCC.C(C)#N.C(C)(=O)OCC
null
2
OCc1c[nH]c(-c2c(F)cccc2F)c1>[Ru](=O)(=O)(=O)[O-].C(CC)[N+](CCC)(CCC)CCC.C(C)#N.C(C)(=O)OCC>O=Cc1c[nH]c(-c2c(F)cccc2F)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-163ff17ba8694624aa224fffbda041ae
OCc1c[nH]c(-c2ccc(C3CCCCC3)cc2)c1>>O=Cc1c[nH]c(-c2ccc(C3CCCCC3)cc2)c1
C1(CCCCC1)C1=CC=C(C=C1)C1=CC(=CN1)CO.C[N+]1(CCOCC1)[O-]>>C1(CCCCC1)C1=CC=C(C=C1)C1=CC(=CN1)C=O
[OH:1][CH2:2][c:3]1[cH:4][nH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([CH:11]3[CH2:12][CH2:13][CH2:14][CH2:15][CH2:16]3)[cH:17][cH:18]2)[cH:19]1>>[O:1]=[CH:2][c:3]1[cH:4][nH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([CH:11]3[CH2:12][CH2:13][CH2:14][CH2:15][CH2:16]3)[cH:17][cH:18]2)[cH:19]1
OCc1c[nH]c(-c2ccc(C3CCCCC3)cc2)c1
O=Cc1c[nH]c(-c2ccc(C3CCCCC3)cc2)c1
null
[Ru](=O)(=O)(=O)[O-].C(CC)[N+](CCC)(CCC)CCC
C(C)#N.C(C)(=O)OCC
Oxidation
Oxidation or Dehydrogenation of Alcohols to Aldehydes and Ketones
41bfa9deea81b465c88ad21fdfb64a2e1ba29490558cf430df132cb98b4a538b
0a03c6724c1862e8f86d4a463afda55b8e067dc6cb42597b472eb7cabc03eda3
c1c[nH]c(-c2ccc(C3CCCCC3)cc2)c1
[OH;D1;+0:1]-[CH2;D2;+0:2]-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[c:7]:1>>[O;H0;D1;+0:1]=[CH;D2;+0:2]-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[c:7]:1
53.4
[{"value": 53.0, "product": "C1(CCCCC1)C1=CC=C(C=C1)C1=CC(=CN1)C=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 53.4, "product": "C1(CCCCC1)C1=CC=C(C=C1)C1=CC(=CN1)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1.5
HOUR
To a solution (35 mL) of [5-(4-cyclohexylphenyl)-1H-pyrrol-3-yl]methanol (1.00 g) in acetonitrile were added tetra-n-propylammonium perruthenate (115 mg), N-methylmorpholine N-oxide (0.60 g) and molecular sieves 4A powder (1.15 g) under ice-cooling. The mixture was stirred at room temperature for 1.5 hr, and the reacti...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Aldehyde
null
null
c1cc[nH]c1.c1ccccc1.C1CCCCC1
null
[Ru](=O)(=O)(=O)[O-].C(CC)[N+](CCC)(CCC)CCC.C(C)#N.C(C)(=O)OCC
null
1.5
OCc1c[nH]c(-c2ccc(C3CCCCC3)cc2)c1>[Ru](=O)(=O)(=O)[O-].C(CC)[N+](CCC)(CCC)CCC.C(C)#N.C(C)(=O)OCC>O=Cc1c[nH]c(-c2ccc(C3CCCCC3)cc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-313288ee16684b83b555dbcdd7c52e28
Cc1ccccc1Br.O=C(O)C(F)(F)Cl>>Cc1ccccc1C(=O)C(F)(F)Cl
ClC(C(=O)O)(F)F.[Mg].II.BrC1=C(C=CC=C1)C.[Cl-].[NH4+]>>ClC(C(=O)C1=C(C=CC=C1)C)(F)F
Br[c:7]1[c:2]([CH3:1])[cH:3][cH:4][cH:5][cH:6]1.O[C:8](=[O:9])[C:10]([F:11])([F:12])[Cl:13]>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1[C:8](=[O:9])[C:10]([F:11])([F:12])[Cl:13]
Cc1ccccc1Br.O=C(O)C(F)(F)Cl
Cc1ccccc1C(=O)C(F)(F)Cl
null
null
C(C)OCC
C-C Coupling
OtherReaction
a68697290bfa0dc1acf39da3d62d1964bdd31d9378f6c352a4a6c9727596388a
e8d827fd3c4c9e4f506ca0217eb2834296a2d5d73d1289088c88acc955f13a34
c1ccccc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[C;D1;H3:5]):[c:6].O-[C;H0;D3;+0:7](=[O;D1;H0:8])-[C:9](-[Cl;D1;H0:10])(-[F;D1;H0:11])-[F;D1;H0:12]>>[C;D1;H3:5]-[c:4](:[c:6]):[c;H0;D3;+0:1](-[C;H0;D3;+0:7](=[O;D1;H0:8])-[C:9](-[Cl;D1;H0:10])(-[F;D1;H0:11])-[F;D1;H0:12]):[c:2]:[c:3]
31.2
[{"value": 31.0, "product": "ClC(C(=O)C1=C(C=CC=C1)C)(F)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 31.2, "product": "ClC(C(=O)C1=C(C=CC=C1)C)(F)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
Magnesium (flake, 6.2 g) was suspended in diethyl ether (10 mL), and iodine (small amount) was added and a solution of 2-bromotoluene (43.26 g) in diethyl ether (100 mL) were slowly added dropwise. After stirring at room temperature for 1 hr, the reaction mixture was added dropwise to a solution of chlorodifluoroacetic...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Carboxylic acid
Ketone
c1ccccc1
c1ccccc1
c1ccccc1
HBr
C(C)OCC
null
1
Cc1ccccc1Br.O=C(O)C(F)(F)Cl>C(C)OCC>Cc1ccccc1C(=O)C(F)(F)Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-458204c058a546459660b75e02c2c7f6
Cc1ccccc1C(=O)C(F)(F)Cl.II>>Cc1ccccc1C(=O)C(F)(F)I
O.C[Si](C)(C)Cl.ClC(C(=O)C1=C(C=CC=C1)C)(F)F.II>>FC(C(=O)C1=C(C=CC=C1)C)(I)F
Cl[C:10]([C:8]([c:7]1[c:2]([CH3:1])[cH:3][cH:4][cH:5][cH:6]1)=[O:9])([F:11])[F:12].I[I:13]>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1[C:8](=[O:9])[C:10]([F:11])([F:12])[I:13]
Cc1ccccc1C(=O)C(F)(F)Cl.II
Cc1ccccc1C(=O)C(F)(F)I
null
[Zn]
C(C)#N
Functional Group Interconversion
OtherReaction
108cc7e043ac402fc9d1d41618d4709c8e5568ce46d961ad76a93e068c18eb94
282cb34e22ed9b87e08e917842a62c2e5c4daf28c7f2abf97c332671d1cb6f2d
c1ccccc1
Cl-[C;H0;D4;+0:1](-[F;D1;H0:2])(-[F;D1;H0:3])-[C:4](=[O;D1;H0:5])-[c:6].I-[I;H0;D1;+0:7]>>[F;D1;H0:2]-[C;H0;D4;+0:1](-[F;D1;H0:3])(-[I;H0;D1;+0:7])-[C:4](=[O;D1;H0:5])-[c:6]
63.7
[{"value": 46.0, "product": "FC(C(=O)C1=C(C=CC=C1)C)(I)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 63.7, "product": "FC(C(=O)C1=C(C=CC=C1)C)(I)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
55
CELSIUS
3
HOUR
To a suspension of zinc (1.6 g) in acetonitrile (40 mL) were added trimethylsilyl chloride (3.1 mL) and 2-chloro-2,2-difluoro-1-(2-methylphenyl)ethanone (4.0 g), and the mixture was stirred at 55° C. for 3 hr. The reaction mixture was allowed to cool to room temperature, iodine (3.5 g) was added, and the mixture was fu...
10.6084/m9.figshare.5104873.v1
null
Tertiary halide.Tertiary halide.Tertiary halide.Ketone
Tertiary halide.Tertiary halide.Tertiary halide
null
null
c1ccccc1
I-
[Zn].C(C)#N
55
3
Cc1ccccc1C(=O)C(F)(F)Cl.II>[Zn].C(C)#N>Cc1ccccc1C(=O)C(F)(F)I
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f899931ab9814f09824145497ed8f6a0
Cc1ccccc1C(=O)C(F)(F)CC(I)[Si](C)(C)C.N>>Cc1ccccc1-c1[nH]ccc1F
FC(C(=O)C1=C(C=CC=C1)C)(CC([Si](C)(C)C)I)F.N>>FC1=C(NC=C1)C1=C(C=CC=C1)C
C[Si](C)(C)[CH:10](I)[CH2:11][C:12](F)([C:8](=O)[c:7]1[c:2]([CH3:1])[cH:3][cH:4][cH:5][cH:6]1)[F:13].[NH3:9]>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1-[c:8]1[nH:9][cH:10][cH:11][c:12]1[F:13]
Cc1ccccc1C(=O)C(F)(F)CC(I)[Si](C)(C)C.N
Cc1ccccc1-c1[nH]ccc1F
null
null
O1CCCC1
Aromatic Heterocycle Formation
OtherReaction
051cdeb87a7dd311937642c85ee3e8d64053c8d8e9e6f70675fc2d89bcd71b45
0282117e50c66ba8a00fb17e01dc7e1944ddf267d0e68532e263d5fd206fd73f
c1ccc(-c2ccc[nH]2)cc1
C-[Si](-C)(-C)-[CH;D3;+0:1](-I)-[CH2;D2;+0:2]-[C;H0;D4;+0:3](-F)(-[F;D1;H0:4])-[C;H0;D3;+0:5](=O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9](-[C;D1;H3:10]):[c:11].[NH3;D0;+0:12]>>[C;D1;H3:10]-[c:9](:[c:11]):[c;H0;D3;+0:6](-[c;H0;D3;+0:5]1:[nH;D2;+0:12]:[cH;D2;+0:1]:[cH;D2;+0:2]:[c;H0;D3;+0:3]:1-[F;D1;H0:4]):[c:7]:[c:8]
78
[{"value": 78.0, "product": "FC1=C(NC=C1)C1=C(C=CC=C1)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
14
HOUR
To a solution (20 mL) of 2,2-difluoro-4-iodo-1-(2-methylphenyl)-4-trimethylsilylbutan-1-one (2.5 g) in tetrahydrofuran was added 28% aqueous ammonia solution (6 mL) and the mixture was stirred at room temperature for 14 hr. The reaction mixture was extracted with ethyl acetate. The extract was washed with saturated bri...
10.6084/m9.figshare.5104873.v1
null
Tertiary halide.Tertiary halide.Secondary halide.Ketone.Silyl protective group
Aromatic halide
null
c1cc[nH]c1
c1ccccc1.c1cc[nH]c1
HF.I-
O1CCCC1
null
14
Cc1ccccc1C(=O)C(F)(F)CC(I)[Si](C)(C)C.N>O1CCCC1>Cc1ccccc1-c1[nH]ccc1F
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-df583e9269374d3c985cdf6acd20a7a8
Cc1ccccc1B(O)O.O=Cc1c[nH]c(Br)c1>>Cc1ccccc1-c1cc(C=O)c[nH]1
COCCOC.BrC1=CC(=CN1)C=O.CC1=C(C=CC=C1)B(O)O.C([O-])([O-])=O.[Na+].[Na+]>>CC1=C(C=CC=C1)C1=CC(=CN1)C=O
OB(O)[c:7]1[c:2]([CH3:1])[cH:3][cH:4][cH:5][cH:6]1.Br[c:8]1[cH:9][c:10]([CH:11]=[O:12])[cH:13][nH:14]1>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1-[c:8]1[cH:9][c:10]([CH:11]=[O:12])[cH:13][nH:14]1
Cc1ccccc1B(O)O.O=Cc1c[nH]c(Br)c1
Cc1ccccc1-c1cc(C=O)c[nH]1
null
null
O
C-C Coupling
Suzuki coupling with boronic acids
b71c1accb23fcf6e808cbf7fdd27a50d721fbf67e253875213e991e29cdecd2f
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc[nH]2)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4](-[C:5]=[O;D1;H0:6]):[c:7]:1.O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11](-[C;D1;H3:12]):[c:13]>>[C;D1;H3:12]-[c:11](:[c:13]):[c;H0;D3;+0:8](-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4](-[C:5]=[O;D1;H0:6]):[c:7]:1):[c:9]:[c:10]
68
[{"value": 68.0, "product": "CC1=C(C=CC=C1)C1=CC(=CN1)C=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 67.6, "product": "CC1=C(C=CC=C1)C1=CC(=CN1)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
105
CELSIUS
null
null
5-Bromo-1H-pyrrole-3-carbaldehyde (100 mg), 2-methylphenylboronic acid (94 mg) and sodium carbonate (146 mg) were suspended in a mixed solvent of 1,2-dimethoxyethane (5 mL) and water (2 mL), and the mixture was sufficiently degassed under a nitrogen atmosphere. Tetrakis(triphenylphosphine)palladium (33 mg) was added, a...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1cc[nH]c1
c1ccccc1.c1cc[nH]c1
c1ccccc1.c1cc[nH]c1
HBr.B
O
105
null
Cc1ccccc1B(O)O.O=Cc1c[nH]c(Br)c1>O>Cc1ccccc1-c1cc(C=O)c[nH]1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a49aea07a2da49c7b258ba354c83128c
O=C1CCC(=O)N1Cl.O=Cc1c[nH]c(-c2ccccc2F)c1>>O=Cc1c[nH]c(-c2ccccc2F)c1Cl
O.FC1=C(C=CC=C1)C1=CC(=CN1)C=O.ClN1C(CCC1=O)=O>>ClC=1C(=CNC1C1=C(C=CC=C1)F)C=O
O=C1CCC(=O)N1[Cl:15].[O:1]=[CH:2][c:3]1[cH:4][nH:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][cH:11][c:12]2[F:13])[cH:14]1>>[O:1]=[CH:2][c:3]1[cH:4][nH:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][cH:11][c:12]2[F:13])[c:14]1[Cl:15]
O=C1CCC(=O)N1Cl.O=Cc1c[nH]c(-c2ccccc2F)c1
O=Cc1c[nH]c(-c2ccccc2F)c1Cl
null
null
CN(C=O)C
Functional Group Interconversion
Chlorination
40ba41cd9c6955f8bb4a47b285f327e8347ac41f3539d665e8b27d9300f356ae
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
c1ccc(-c2ccc[nH]2)cc1
O=C1-C-C-C(=O)-N-1-[Cl;H0;D1;+0:1].[O;D1;H0:2]=[C:3]-[c:4]1:[c:5]:[#7;a:6]:[c:7](-[c:8]):[cH;D2;+0:9]:1>>[Cl;H0;D1;+0:1]-[c;H0;D3;+0:9]1:[c:4](-[C:3]=[O;D1;H0:2]):[c:5]:[#7;a:6]:[c:7]:1-[c:8]
46.5
[{"value": 46.0, "product": "ClC=1C(=CNC1C1=C(C=CC=C1)F)C=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 46.5, "product": "ClC=1C(=CNC1C1=C(C=CC=C1)F)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
2
HOUR
To a solution (15 mL) of 5-(2-fluorophenyl)-1H-pyrrole-3-carbaldehyde (1.0 g) in N,N-dimethylformamide was added N-chlorosuccinimide (0.71 g) at 0° C., and the mixture was stirred at 60° C. for 2 hr. The mixture was cooled to room temperature, water was added and the mixture was extracted with ethyl acetate. The extrac...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
C1CCNC1.c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccccc1
HO-
CN(C=O)C
60
2
O=C1CCC(=O)N1Cl.O=Cc1c[nH]c(-c2ccccc2F)c1>CN(C=O)C>O=Cc1c[nH]c(-c2ccccc2F)c1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5e83aa001928401983a83acc4bd6dd91
O=Cc1c[nH]c(-c2ccccc2F)c1>>O=Cc1c[nH]c(-c2ccccc2F)c1F
C(O)([O-])=O.[Na+].FC1=C(C=CC=C1)C1=CC(=CN1)C=O.[O-]S(=O)(=O)C(F)(F)F.ClC1=[N+](C(=CC=C1)Cl)F>>FC=1C(=CNC1C1=C(C=CC=C1)F)C=O
[O:1]=[CH:2][c:3]1[cH:4][nH:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][cH:11][c:12]2[F:13])[cH:14]1>>[O:1]=[CH:2][c:3]1[cH:4][nH:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][cH:11][c:12]2[F:13])[c:14]1[F:15]
O=Cc1c[nH]c(-c2ccccc2F)c1
O=Cc1c[nH]c(-c2ccccc2F)c1F
null
null
O1CCCC1
Functional Group Addition
Aromatic fluorination
4048bac0b4c21eb6e694a585c03c487c6380befb41bf01d9388a95029c960e33
0a2f22058f27970cef4a98a778644dbe9c44e91f66c74cd24db321993177608a
c1ccc(-c2ccc[nH]2)cc1
[O;D1;H0:1]=[C:2]-[c:3]1:[c:4]:[#7;a:5]:[c:6](-[c:7]):[cH;D2;+0:8]:1>>[F;D1;H0:9]-[c;H0;D3;+0:8]1:[c:3](-[C:2]=[O;D1;H0:1]):[c:4]:[#7;a:5]:[c:6]:1-[c:7]
13
[{"value": 13.0, "product": "FC=1C(=CNC1C1=C(C=CC=C1)F)C=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 12.7, "product": "FC=1C(=CNC1C1=C(C=CC=C1)F)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
To a solution (60 mL) of 5-(2-fluorophenyl)-1H-pyrrole-3-carbaldehyde (3.1 g) in tetrahydrofuran was added 2,6-dichloro-N-fluoropyridinium triflate (5.6 g) at 0° C., and the mixture was stirred at the same temperature for 2 hr. Saturated aqueous sodium hydrogencarbonate solution was added to the reaction mixture, and t...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccccc1
Other
O1CCCC1
null
2
O=Cc1c[nH]c(-c2ccccc2F)c1>O1CCCC1>O=Cc1c[nH]c(-c2ccccc2F)c1F
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-88d492a5e242401fbc7ef19574437c3b
O=[N+]([O-])O.Oc1ncccc1C(F)(F)F>>O=[N+]([O-])c1cnc(O)c(C(F)(F)F)c1
OC1=NC=CC=C1C(F)(F)F.S(O)(O)(=O)=O.[N+](=O)(O)[O-]>>[N+](=O)([O-])C=1C=C(C(=NC1)O)C(F)(F)F
O[N+:2](=[O:1])[O-:3].[cH:4]1[cH:5][n:6][c:7]([OH:8])[c:9]([C:10]([F:11])([F:12])[F:13])[cH:14]1>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][n:6][c:7]([OH:8])[c:9]([C:10]([F:11])([F:12])[F:13])[cH:14]1
O=[N+]([O-])O.Oc1ncccc1C(F)(F)F
O=[N+]([O-])c1cnc(O)c(C(F)(F)F)c1
null
null
null
Functional Group Addition
Aromatic nitration with HNO3
cb3ba0bb7f4ff246f608a5c967bfb512792a47826af0eb60d49c2f2aea6e8ead
ddce49825c02b8965f10c8d99e3c841d26e1f136da6037b417c09313e6d73097
c1ccncc1
O-[N+;H0;D3:1](-[O;-;D1;H0:2])=[O;D1;H0:3].[#7;a:4]1:[c:5]:[cH;D2;+0:6]:[c:7]:[c:8]:[c:9]:1>>[O;-;D1;H0:2]-[N+;H0;D3:1](=[O;D1;H0:3])-[c;H0;D3;+0:6]1:[c:7]:[c:8]:[c:9]:[#7;a:4]:[c:5]:1
69
[{"value": 69.0, "product": "[N+](=O)([O-])C=1C=C(C(=NC1)O)C(F)(F)F", "details": "PERCENTYIELD", "is_desired": false}]
50
CELSIUS
5
MINUTE
2-Hydroxy-3-(trifluoromethyl)pyridine (3.0 g) was added to conc. sulfuric acid (18 mL) under ice-cooling, and the mixture was stirred at the same temperature for 5 min. Fuming nitric acid (90-95%, 7 mL) was added dropwise over 5 min, and the mixture was allowed to return to room temperature over 2 hr, heated to 50° C. ...
10.6084/m9.figshare.5104873.v1
null
Nitrate
Nitro group
c1ccncc1
c1ccncc1
c1ccncc1
HO-
null
50
0.083333
O=[N+]([O-])O.Oc1ncccc1C(F)(F)F>>O=[N+]([O-])c1cnc(O)c(C(F)(F)F)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4652682c7d4a4d75a1ee469f5d8fd15d
O=P(Cl)(Cl)Cl.O=[N+]([O-])c1cnc(O)c(C(F)(F)F)c1>>O=[N+]([O-])c1cnc(Cl)c(C(F)(F)F)c1
[N+](=O)([O-])C=1C=C(C(=NC1)O)C(F)(F)F.P(Cl)(Cl)(Cl)(Cl)Cl.P(=O)(Cl)(Cl)Cl>>ClC1=NC=C(C=C1C(F)(F)F)[N+](=O)[O-]
O=P(Cl)(Cl)[Cl:8].O[c:7]1[n:6][cH:5][c:4]([N+:2](=[O:1])[O-:3])[cH:14][c:9]1[C:10]([F:11])([F:12])[F:13]>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][n:6][c:7]([Cl:8])[c:9]([C:10]([F:11])([F:12])[F:13])[cH:14]1
O=P(Cl)(Cl)Cl.O=[N+]([O-])c1cnc(O)c(C(F)(F)F)c1
O=[N+]([O-])c1cnc(Cl)c(C(F)(F)F)c1
null
null
null
Functional Group Interconversion
Alcohol to chloride_POCl3_ortho
ab85b19a1f19bdb0596b983dc6471067aedf5e7b894e737e6d16cd077bd81b42
e71580a8ffadb7b2717ecd7d68c1d3c0ca161ba5e6a787a49dad5a1359adc993
c1ccncc1
Cl-P(-Cl)(=O)-[Cl;H0;D1;+0:1].O-[c;H0;D3;+0:2](:[#7;a:3]:[c:4]):[c:5](-[C:6](-[F;D1;H0:7])(-[F;D1;H0:8])-[F;D1;H0:9]):[c:10]>>[Cl;H0;D1;+0:1]-[c;H0;D3;+0:2](:[#7;a:3]:[c:4]):[c:5](-[C:6](-[F;D1;H0:7])(-[F;D1;H0:8])-[F;D1;H0:9]):[c:10]
77
[{"value": 77.0, "product": "ClC1=NC=C(C=C1C(F)(F)F)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 76.6, "product": "ClC1=NC=C(C=C1C(F)(F)F)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
90
CELSIUS
3
HOUR
A mixture of 5-nitro-3-(trifluoromethyl)pyridin-2-ol (2.65 g), phosphorus pentachloride (3.17 g) and phosphorus oxychloride (1.5 mL) was stirred at 90° C. for 3 hr. After cooling to room temperature, the reaction mixture was poured into ice, and the mixture was extracted with ethyl acetate. The extract was washed with ...
10.6084/m9.figshare.5104873.v1
null
Aromatic alcohol
Aromatic halide
c1ccncc1
c1ccncc1
c1ccncc1
HCl
null
90
3
O=P(Cl)(Cl)Cl.O=[N+]([O-])c1cnc(O)c(C(F)(F)F)c1>>O=[N+]([O-])c1cnc(Cl)c(C(F)(F)F)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-83e3531e09504611a6037eefb446e02f
O=[N+]([O-])c1cnc(Cl)c(C(F)(F)F)c1>>Nc1cnc(Cl)c(C(F)(F)F)c1
[Cl-].[NH4+].O.ClC1=NC=C(C=C1C(F)(F)F)[N+](=O)[O-]>>ClC1=C(C=C(C=N1)N)C(F)(F)F
O=[N+:1]([O-])[c:2]1[cH:3][n:4][c:5]([Cl:6])[c:7]([C:8]([F:9])([F:10])[F:11])[cH:12]1>>[NH2:1][c:2]1[cH:3][n:4][c:5]([Cl:6])[c:7]([C:8]([F:9])([F:10])[F:11])[cH:12]1
O=[N+]([O-])c1cnc(Cl)c(C(F)(F)F)c1
Nc1cnc(Cl)c(C(F)(F)F)c1
null
null
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccncc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]:[#7;a:5]:[c:6]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]:[#7;a:5]:[c:6]
65
[{"value": 65.0, "product": "ClC1=C(C=C(C=N1)N)C(F)(F)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 64.0, "product": "ClC1=C(C=C(C=N1)N)C(F)(F)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
5
MINUTE
Reduced iron (1.3 g) and ammonium chloride (2.1 g) were added to water (40 mL), and the mixture was stirred at room temperature for 5 min. A solution of 2-chloro-5-nitro-3-(trifluoromethyl)pyridine (1.8 g) in methanol (40 mL) was added, and the mixture was stirred at room temperature for 1 hr. Reduced iron (2.3 g) was ...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccncc1
Other
CO
null
0.083333
O=[N+]([O-])c1cnc(Cl)c(C(F)(F)F)c1>CO>Nc1cnc(Cl)c(C(F)(F)F)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-fd4e953545234f1ca82bae093906a7d8
Cl.Nc1cnc(Cl)c(C(F)(F)F)c1.O=S=O>>O=S(=O)(Cl)c1cnc(Cl)c(C(F)(F)F)c1
S(=O)=O.N(=O)[O-].[Na+].ClC1=C(C=C(C=N1)N)C(F)(F)F.Cl.Cl>>ClC1=C(C=C(C=N1)S(=O)(=O)Cl)C(F)(F)F
[ClH:4].N[c:5]1[cH:6][n:7][c:8]([Cl:9])[c:10]([C:11]([F:12])([F:13])[F:14])[cH:15]1.[O:1]=[S:2]=[O:3]>>[O:1]=[S:2](=[O:3])([Cl:4])[c:5]1[cH:6][n:7][c:8]([Cl:9])[c:10]([C:11]([F:12])([F:13])[F:14])[cH:15]1
Cl.Nc1cnc(Cl)c(C(F)(F)F)c1.O=S=O
O=S(=O)(Cl)c1cnc(Cl)c(C(F)(F)F)c1
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
d44a4364e5511e440a48fb914cbd59017338faff430f0e7127e14fae8b0eff0a
49dcc8f7b4471977f8fe724b4dd774612c303d853f75a373d5b25cc7ccd4c205
c1ccncc1
N-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[#7;a:5]:[c:6]:1.[ClH;D0;+0:7].[O;D1;H0:8]=[S;H0;D2;+0:9]=[O;D1;H0:10]>>[Cl;H0;D1;+0:7]-[S;H0;D4;+0:9](=[O;D1;H0:8])(=[O;D1;H0:10])-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[#7;a:5]:[c:6]:1
27
[{"value": 27.0, "product": "ClC1=C(C=C(C=N1)S(=O)(=O)Cl)C(F)(F)F", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
Under ice-cooling, thionyl chloride (4 mL) was added dropwise over 20 min to water (27 mL). The mixture was stirred at room temperature for 12 hr to give a sulfur dioxide-containing solution. Separately, 6-chloro-5-(trifluoromethyl)pyridine-3-amine (1.14 g) was added to concentrated hydrochloric acid (9 mL) with stirri...
10.6084/m9.figshare.5104873.v1
null
Primary amine
Sulfonyl halide
c1ccncc1
c1ccncc1
c1ccncc1
Other
O
null
null
Cl.Nc1cnc(Cl)c(C(F)(F)F)c1.O=S=O>O>O=S(=O)(Cl)c1cnc(Cl)c(C(F)(F)F)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8124e260b99f48bdb6170f7787b35dd9
Cc1nc(Cl)ccc1N.Cl.O=S=O>>Cc1nc(Cl)ccc1S(=O)(=O)Cl
S(=O)=O.N(=O)[O-].[Na+].Cl.NC=1C=CC(=NC1C)Cl>>ClC1=CC=C(C(=N1)C)S(=O)(=O)Cl
N[c:8]1[c:2]([CH3:1])[n:3][c:4]([Cl:5])[cH:6][cH:7]1.[ClH:12].[S:9](=[O:10])=[O:11]>>[CH3:1][c:2]1[n:3][c:4]([Cl:5])[cH:6][cH:7][c:8]1[S:9](=[O:10])(=[O:11])[Cl:12]
Cc1nc(Cl)ccc1N.Cl.O=S=O
Cc1nc(Cl)ccc1S(=O)(=O)Cl
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
d44a4364e5511e440a48fb914cbd59017338faff430f0e7127e14fae8b0eff0a
49dcc8f7b4471977f8fe724b4dd774612c303d853f75a373d5b25cc7ccd4c205
c1ccncc1
N-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[#7;a:5]:[c:6]:1-[C;D1;H3:7].[ClH;D0;+0:8].[O;D1;H0:9]=[S;H0;D2;+0:10]=[O;D1;H0:11]>>[C;D1;H3:7]-[c:6]1:[#7;a:5]:[c:4]:[c:3]:[c:2]:[c;H0;D3;+0:1]:1-[S;H0;D4;+0:10](-[Cl;H0;D1;+0:8])(=[O;D1;H0:9])=[O;D1;H0:11]
67
[{"value": 67.0, "product": "ClC1=CC=C(C(=N1)C)S(=O)(=O)Cl", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
Under ice-cooling, thionyl chloride (4 mL) was added dropwise to water (24 mL) over 20 min. The mixture was stirred at room temperature for 12 hr to give a sulfur dioxide-containing solution. Separately, to the concentrated hydrochloric acid (6 mL) was added 5-amino-2-chloro-6-methylpyridine (1.0 g) with stirring under...
10.6084/m9.figshare.5104873.v1
null
Primary amine
Sulfonyl halide
c1ccncc1
c1ccncc1
c1ccncc1
Other
O
null
null
Cc1nc(Cl)ccc1N.Cl.O=S=O>O>Cc1nc(Cl)ccc1S(=O)(=O)Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-24fc362e9e4f48f08ac10fb8dd7b4243
COC(=O)c1c[nH]c(-c2ccccc2)c1F.O=S(=O)(Cl)c1cccnc1>>COC(=O)c1cn(S(=O)(=O)c2cccnc2)c(-c2ccccc2)c1F
Cl.N1=CC(=CC=C1)S(=O)(=O)Cl.C1COCCOCCOCCOCCO1.FC=1C(=CNC1C1=CC=CC=C1)C(=O)OC.[H-].[Na+]>>FC=1C(=CN(C1C1=CC=CC=C1)S(=O)(=O)C=1C=NC=CC1)C(=O)OC
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][nH:7][c:17](-[c:18]2[cH:19][cH:20][cH:21][cH:22][cH:23]2)[c:24]1[F:25].Cl[S:8](=[O:9])(=[O:10])[c:11]1[cH:12][cH:13][cH:14][n:15][cH:16]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][n:7]([S:8](=[O:9])(=[O:10])[c:11]2[cH:12][cH:13][cH:14][n:15][cH:16]2)[c:17](-[c:18]2[cH:19][cH:20][cH:21...
COC(=O)c1c[nH]c(-c2ccccc2)c1F.O=S(=O)(Cl)c1cccnc1
COC(=O)c1cn(S(=O)(=O)c2cccnc2)c(-c2ccccc2)c1F
null
null
O1CCCC1.O
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8].[#8:9]-[C:10](=[O;D1;H0:11])-[c:12]1:[c:13]:[c:14](-[c:15]):[nH;D2;+0:16]:[c:17]:1>>[#8:9]-[C:10](=[O;D1;H0:11])-[c:12]1:[c:13]:[c:14](-[c:15]):[n;H0;D3;+0:16](-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8])...
73
[{"value": 73.0, "product": "FC=1C(=CN(C1C1=CC=CC=C1)S(=O)(=O)C=1C=NC=CC1)C(=O)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 72.9, "product": "FC=1C(=CN(C1C1=CC=CC=C1)S(=O)(=O)C=1C=NC=CC1)C(=O)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
By a similar reaction as in Reference Example 36 and using methyl 4-fluoro-5-phenyl-1H-pyrrole-3-carboxylate (172 mg), the title compound was obtained as a colorless solid (yield 206 mg, 73%). More specifically, to a solution of methyl 4-fluoro-5-phenyl-1H-pyrrole-3-carboxylate (172 mg) in tetrahydrofuran (10 mL) was a...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccncc1.c1ccccc1
HCl
O1CCCC1.O
null
0.25
COC(=O)c1c[nH]c(-c2ccccc2)c1F.O=S(=O)(Cl)c1cccnc1>O1CCCC1.O>COC(=O)c1cn(S(=O)(=O)c2cccnc2)c(-c2ccccc2)c1F
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-45007b94ab8d42eabd48f68260c7a547
COC(=O)c1cn(S(=O)(=O)c2cccnc2)c(-c2ccccc2)c1F>>O=Cc1cn(S(=O)(=O)c2cccnc2)c(-c2ccccc2)c1F
O.[H-].C(C(C)C)[Al+]CC(C)C.FC=1C(=CN(C1C1=CC=CC=C1)S(=O)(=O)C=1C=NC=CC1)C(=O)OC.C(C)(=O)OCC>>FC=1C(=CN(C1C1=CC=CC=C1)S(=O)(=O)C=1C=NC=CC1)C=O
CO[C:2](=[O:1])[c:3]1[cH:4][n:5]([S:6](=[O:7])(=[O:8])[c:9]2[cH:10][cH:11][cH:12][n:13][cH:14]2)[c:15](-[c:16]2[cH:17][cH:18][cH:19][cH:20][cH:21]2)[c:22]1[F:23]>>[O:1]=[CH:2][c:3]1[cH:4][n:5]([S:6](=[O:7])(=[O:8])[c:9]2[cH:10][cH:11][cH:12][n:13][cH:14]2)[c:15](-[c:16]2[cH:17][cH:18][cH:19][cH:20][cH:21]2)[c:22]1[F:23...
COC(=O)c1cn(S(=O)(=O)c2cccnc2)c(-c2ccccc2)c1F
O=Cc1cn(S(=O)(=O)c2cccnc2)c(-c2ccccc2)c1F
null
null
O1CCCC1.C1(=CC=CC=C1)C
Reduction
OtherReaction
ec1c6c64dd9be73981e5a6c952ab740869d298b20e87e097e88e1179cc5bc6dc
33ddc7b9457742ba0a376f08a972e4f33779267f6f1fe15e3be786427ae9f4ec
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[c:5]:[#7;a:6](-[#16:7]):[c:8]:1>>[#16:7]-[#7;a:6]1:[c:5]:[c:4]:[c:3](-[CH;D2;+0:1]=[O;D1;H0:2]):[c:8]:1
67.1
[{"value": 67.0, "product": "FC=1C(=CN(C1C1=CC=CC=C1)S(=O)(=O)C=1C=NC=CC1)C=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 67.1, "product": "FC=1C(=CN(C1C1=CC=CC=C1)S(=O)(=O)C=1C=NC=CC1)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
null
null
Under a nitrogen atmosphere, a solution of methyl 4-fluoro-5-phenyl-1-(pyridin-3-ylsulfonyl)-1H-pyrrole-3-carboxylate (200 mg) in tetrahydrofuran (10 mL) was cooled to −78° C., and a 1.5 mol/L solution (1.85 mL) of diisobutylaluminum hydride in toluene was added with stirring. After stirring at the same temperature for...
10.6084/m9.figshare.5104873.v1
null
Ester
Aldehyde
null
null
c1cc[nH]c1.c1ccncc1.c1ccccc1
HO-
O1CCCC1.C1(=CC=CC=C1)C
0
null
COC(=O)c1cn(S(=O)(=O)c2cccnc2)c(-c2ccccc2)c1F>O1CCCC1.C1(=CC=CC=C1)C>O=Cc1cn(S(=O)(=O)c2cccnc2)c(-c2ccccc2)c1F
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-79e4e84da2e64437811dc45c52d3b3eb
O=Cc1c[nH]c(-c2c(F)cccc2F)c1.O=S(=O)(Cl)c1cccnc1>>O=Cc1cc(-c2c(F)cccc2F)n(S(=O)(=O)c2cccnc2)c1
Cl.N1=CC(=CC=C1)S(=O)(=O)Cl.C1COCCOCCOCCOCCO1.FC1=C(C(=CC=C1)F)C1=CC(=CN1)C=O.[H-].[Na+]>>FC1=C(C(=CC=C1)F)C1=CC(=CN1S(=O)(=O)C=1C=NC=CC1)C=O
[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[c:7]([F:8])[cH:9][cH:10][cH:11][c:12]2[F:13])[nH:14][cH:24]1.Cl[S:15](=[O:16])(=[O:17])[c:18]1[cH:19][cH:20][cH:21][n:22][cH:23]1>>[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[c:7]([F:8])[cH:9][cH:10][cH:11][c:12]2[F:13])[n:14]([S:15](=[O:16])(=[O:17])[c:18]2[cH:19][cH:20][cH:21][n:22][cH...
O=Cc1c[nH]c(-c2c(F)cccc2F)c1.O=S(=O)(Cl)c1cccnc1
O=Cc1cc(-c2c(F)cccc2F)n(S(=O)(=O)c2cccnc2)c1
null
null
O1CCCC1.[Cl-].[Na+].O
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8].[O;D1;H0:9]=[C:10]-[c:11]1:[c:12]:[nH;D2;+0:13]:[c:14](-[c:15]):[c:16]:1>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8])-[n;H0;D3;+0:13]1:[c:12]:[c:11](-[C:10]=[O;D1;H0:9]):[c:16]:[c:14]:1-[c:15]
84
[{"value": 84.0, "product": "FC1=C(C(=CC=C1)F)C1=CC(=CN1S(=O)(=O)C=1C=NC=CC1)C=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 83.6, "product": "FC1=C(C(=CC=C1)F)C1=CC(=CN1S(=O)(=O)C=1C=NC=CC1)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
To a solution of 5-(2,6-difluorophenyl)-1H-pyrrole-3-carbaldehyde (420 mg) in tetrahydrofuran (42 mL) was added sodium hydride (60% in oil, 244 mg) at room temperature and the mixture was stirred for 30 min. 15-Crown-5 (1.34 g) was added dropwise and the mixture was stirred for 30 min. 3-Pyridylsulfonyl chloride hydroc...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccccc1.c1ccncc1
HCl
O1CCCC1.[Cl-].[Na+].O
null
0.5
O=Cc1c[nH]c(-c2c(F)cccc2F)c1.O=S(=O)(Cl)c1cccnc1>O1CCCC1.[Cl-].[Na+].O>O=Cc1cc(-c2c(F)cccc2F)n(S(=O)(=O)c2cccnc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0e50b74befd8425a8fb7dd35a1328ccc
O=Cc1c[nH]c(-c2ccc(C3CCCCC3)cc2)c1.O=S(=O)(Cl)c1cccnc1>>O=Cc1cc(-c2ccc(C3CCCCC3)cc2)n(S(=O)(=O)c2cccnc2)c1
[H-].[Na+].C1(CCCCC1)C1=CC=C(C=C1)C1=CC(=CN1)C=O.N1=CC(=CC=C1)S(=O)(=O)Cl>>C1(CCCCC1)C1=CC=C(C=C1)C1=CC(=CN1S(=O)(=O)C=1C=NC=CC1)C=O
[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][c:9]([CH:10]3[CH2:11][CH2:12][CH2:13][CH2:14][CH2:15]3)[cH:16][cH:17]2)[nH:18][cH:28]1.Cl[S:19](=[O:20])(=[O:21])[c:22]1[cH:23][cH:24][cH:25][n:26][cH:27]1>>[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][c:9]([CH:10]3[CH2:11][CH2:12][CH2:13][CH2:14][CH2:15]3)[cH:16][...
O=Cc1c[nH]c(-c2ccc(C3CCCCC3)cc2)c1.O=S(=O)(Cl)c1cccnc1
O=Cc1cc(-c2ccc(C3CCCCC3)cc2)n(S(=O)(=O)c2cccnc2)c1
null
null
O1CCCC1
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cccnc1)n1cccc1-c1ccc(C2CCCCC2)cc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8].[O;D1;H0:9]=[C:10]-[c:11]1:[c:12]:[nH;D2;+0:13]:[c:14](-[c:15]):[c:16]:1>>[O;D1;H0:9]=[C:10]-[c:11]1:[c:12]:[n;H0;D3;+0:13](-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8]):[c:14](-[c:15]):[c:16]:1
98.2
[{"value": 97.0, "product": "C1(CCCCC1)C1=CC=C(C=C1)C1=CC(=CN1S(=O)(=O)C=1C=NC=CC1)C=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 98.2, "product": "C1(CCCCC1)C1=CC=C(C=C1)C1=CC(=CN1S(=O)(=O)C=1C=NC=CC1)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
20
MINUTE
Sodium hydride (60% in oil, 68 mg) was added to a solution of 5-(4-cyclohexylphenyl)-1H-pyrrole-3-carbaldehyde (0.17 g) in tetrahydrofuran (12 mL) at room temperature. The mixture was stirred for 20 min, 3-pyridinesulfonyl chloride (0.19 g) was added, and the mixture was stirred at room temperature for 3 hr. The reacti...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccccc1.C1CCCCC1.c1ccncc1
HCl
O1CCCC1
null
0.333333
O=Cc1c[nH]c(-c2ccc(C3CCCCC3)cc2)c1.O=S(=O)(Cl)c1cccnc1>O1CCCC1>O=Cc1cc(-c2ccc(C3CCCCC3)cc2)n(S(=O)(=O)c2cccnc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d9c6dc74a8624dce83e08f84ae62bccf
O=Cc1c[nH]c(-c2ccccc2F)c1.O=S(=O)(Cl)c1ccc(Cl)nc1>>O=Cc1cc(-c2ccccc2F)n(S(=O)(=O)c2ccc(Cl)nc2)c1
FC1=C(C=CC=C1)C1=CC(=CN1)C=O.ClC1=CC=C(C=N1)S(=O)(=O)Cl>>ClC1=CC=C(C=N1)S(=O)(=O)N1C=C(C=C1C1=C(C=CC=C1)F)C=O
[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][cH:9][cH:10][c:11]2[F:12])[nH:13][cH:24]1.Cl[S:14](=[O:15])(=[O:16])[c:17]1[cH:18][cH:19][c:20]([Cl:21])[n:22][cH:23]1>>[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][cH:9][cH:10][c:11]2[F:12])[n:13]([S:14](=[O:15])(=[O:16])[c:17]2[cH:18][cH:19][c:20]([Cl:21])[n:22][...
O=Cc1c[nH]c(-c2ccccc2F)c1.O=S(=O)(Cl)c1ccc(Cl)nc1
O=Cc1cc(-c2ccccc2F)n(S(=O)(=O)c2ccc(Cl)nc2)c1
null
null
null
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8].[O;D1;H0:9]=[C:10]-[c:11]1:[c:12]:[nH;D2;+0:13]:[c:14](-[c:15]):[c:16]:1>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8])-[n;H0;D3;+0:13]1:[c:12]:[c:11](-[C:10]=[O;D1;H0:9]):[c:16]:[c:14]:1-[c:15]
66
[{"value": 66.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a similar reaction as in Reference Example 65 and using 5-(2-fluorophenyl)-1H-pyrrole-3-carbaldehyde (893 mg) and 6-chloropyridine-3-sulfonyl chloride (1.30 g), the title compound was obtained as a pale-red solid (yield 1.14 g, 66%). More specifically, 5-(2-fluorophenyl)-1H-pyrrole-3-carbaldehyde (893 mg) was dissol...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccccc1.c1ccncc1
HCl
null
null
null
O=Cc1c[nH]c(-c2ccccc2F)c1.O=S(=O)(Cl)c1ccc(Cl)nc1>>O=Cc1cc(-c2ccccc2F)n(S(=O)(=O)c2ccc(Cl)nc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-18e1e79248804e76927271685b61fe9c
O=Cc1c[nH]c(-c2ccccc2F)c1.O=S(=O)(Cl)c1ccc(Cl)nc1>>O=Cc1cc(-c2ccccc2F)n(S(=O)(=O)c2ccc(Cl)nc2)c1
ClC1=CC=C(C=N1)S(=O)(=O)Cl.[H-].[Na+].FC1=C(C=CC=C1)C1=CC(=CN1)C=O.C1COCCOCCOCCOCCO1>>ClC1=CC=C(C=N1)S(=O)(=O)N1C=C(C=C1C1=C(C=CC=C1)F)C=O
[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][cH:9][cH:10][c:11]2[F:12])[nH:13][cH:24]1.Cl[S:14](=[O:15])(=[O:16])[c:17]1[cH:18][cH:19][c:20]([Cl:21])[n:22][cH:23]1>>[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][cH:9][cH:10][c:11]2[F:12])[n:13]([S:14](=[O:15])(=[O:16])[c:17]2[cH:18][cH:19][c:20]([Cl:21])[n:22][...
O=Cc1c[nH]c(-c2ccccc2F)c1.O=S(=O)(Cl)c1ccc(Cl)nc1
O=Cc1cc(-c2ccccc2F)n(S(=O)(=O)c2ccc(Cl)nc2)c1
null
null
O1CCCC1.O
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8].[O;D1;H0:9]=[C:10]-[c:11]1:[c:12]:[nH;D2;+0:13]:[c:14](-[c:15]):[c:16]:1>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8])-[n;H0;D3;+0:13]1:[c:12]:[c:11](-[C:10]=[O;D1;H0:9]):[c:16]:[c:14]:1-[c:15]
66.2
[{"value": 66.0, "product": "ClC1=CC=C(C=N1)S(=O)(=O)N1C=C(C=C1C1=C(C=CC=C1)F)C=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 66.2, "product": "ClC1=CC=C(C=N1)S(=O)(=O)N1C=C(C=C1C1=C(C=CC=C1)F)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
By a similar reaction as in Reference Example 65 and using 5-(2-fluorophenyl)-1H-pyrrole-3-carbaldehyde (893 mg) and 6-chloropyridine-3-sulfonyl chloride (1.30 g), the title compound was obtained as a pale-red solid (yield 1.14 g, 66%). More specifically, 5-(2-fluorophenyl)-1H-pyrrole-3-carbaldehyde (893 mg) was dissol...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccccc1.c1ccncc1
HCl
O1CCCC1.O
null
0.25
O=Cc1c[nH]c(-c2ccccc2F)c1.O=S(=O)(Cl)c1ccc(Cl)nc1>O1CCCC1.O>O=Cc1cc(-c2ccccc2F)n(S(=O)(=O)c2ccc(Cl)nc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-25fb8434bdeb463e91b2ef83263f66cc
CB(O)O.O=Cc1cc(-c2ccccc2F)n(S(=O)(=O)c2ccc(Cl)nc2)c1>>Cc1ccc(S(=O)(=O)n2cc(C=O)cc2-c2ccccc2F)cn1
C(O)([O-])=O.[Na+].ClC1=CC=C(C=N1)S(=O)(=O)N1C=C(C=C1C1=C(C=CC=C1)F)C=O.CB(O)O.C([O-])([O-])=O.[K+].[K+]>>FC1=C(C=CC=C1)C1=CC(=CN1S(=O)(=O)C=1C=NC(=CC1)C)C=O
OB(O)[CH3:1].Cl[c:2]1[cH:3][cH:4][c:5]([S:6](=[O:7])(=[O:8])[n:9]2[cH:10][c:11]([CH:12]=[O:13])[cH:14][c:15]2-[c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[F:22])[cH:23][n:24]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([S:6](=[O:7])(=[O:8])[n:9]2[cH:10][c:11]([CH:12]=[O:13])[cH:14][c:15]2-[c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[...
CB(O)O.O=Cc1cc(-c2ccccc2F)n(S(=O)(=O)c2ccc(Cl)nc2)c1
Cc1ccc(S(=O)(=O)n2cc(C=O)cc2-c2ccccc2F)cn1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O1CCOCC1
C-C Coupling
Suzuki coupling with boronic acids
e6427a06cf763f629ade010ec8edb6d572dcafeb9186c64e3948e154bc0e8e0d
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[CH3;D1;+0:6]>>[CH3;D1;+0:6]-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5]
39
[{"value": 39.0, "product": "FC1=C(C=CC=C1)C1=CC(=CN1S(=O)(=O)C=1C=NC(=CC1)C)C=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 38.9, "product": "FC1=C(C=CC=C1)C1=CC(=CN1S(=O)(=O)C=1C=NC(=CC1)C)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
3
DAY
Under an argon atmosphere, a mixture of 1-[(6-chloropyridin-3-yl)sulfonyl]-5-(2-fluorophenyl)-1H-pyrrole-3-carbaldehyde (365 mg), methylboronic acid (90 mg), tetrakis(triphenylphosphine)palladium (116 mg), potassium carbonate (691 mg) and 1,4-dioxane (25 mL) was stirred at 80° C. for 3 days. The reaction mixture was po...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccncc1
c1ccncc1
c1ccncc1.c1cc[nH]c1.c1ccccc1
HCl.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1
80
72
CB(O)O.O=Cc1cc(-c2ccccc2F)n(S(=O)(=O)c2ccc(Cl)nc2)c1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1>Cc1ccc(S(=O)(=O)n2cc(C=O)cc2-c2ccccc2F)cn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-eee68b78c04747ad87d7082d10851e72
O=Cc1c[nH]c(-c2ccccc2F)c1.O=S(=O)(Cl)c1ccccn1>>O=Cc1cc(-c2ccccc2F)n(S(=O)(=O)c2ccccn2)c1
FC1=C(C=CC=C1)C1=CC(=CN1)C=O.N1=C(C=CC=C1)S(=O)(=O)Cl>>FC1=C(C=CC=C1)C1=CC(=CN1S(=O)(=O)C1=NC=CC=C1)C=O
[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][cH:9][cH:10][c:11]2[F:12])[nH:13][cH:23]1.Cl[S:14](=[O:15])(=[O:16])[c:17]1[cH:18][cH:19][cH:20][cH:21][n:22]1>>[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][cH:9][cH:10][c:11]2[F:12])[n:13]([S:14](=[O:15])(=[O:16])[c:17]2[cH:18][cH:19][cH:20][cH:21][n:22]2)[cH:23]1
O=Cc1c[nH]c(-c2ccccc2F)c1.O=S(=O)(Cl)c1ccccn1
O=Cc1cc(-c2ccccc2F)n(S(=O)(=O)c2ccccn2)c1
null
null
null
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1ccccn1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[#7;a:6]:[c:7].[O;D1;H0:8]=[C:9]-[c:10]1:[c:11]:[nH;D2;+0:12]:[c:13](-[c:14]):[c:15]:1>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[c:4](:[c:5]):[#7;a:6]:[c:7])-[n;H0;D3;+0:12]1:[c:11]:[c:10](-[C:9]=[O;D1;H0:8]):[c:15]:[c:13]:1-[c:14]
55
[{"value": 55.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a similar reaction as in Reference Example 65 and using 5-(2-fluorophenyl)-1H-pyrrole-3-carbaldehyde (190 mg) and pyridine-2-sulfonyl chloride (231 mg), the title compound was obtained as a pale-red solid (yield 183 mg, 55%). Conditions: See reaction.notes.procedure_details. Workup: By a similar reaction as in Refer...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccccc1.c1ccncc1
HCl
null
null
null
O=Cc1c[nH]c(-c2ccccc2F)c1.O=S(=O)(Cl)c1ccccn1>>O=Cc1cc(-c2ccccc2F)n(S(=O)(=O)c2ccccn2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7c914aeb94624ef5875a34038c36d1db
Cn1cc(S(=O)(=O)Cl)cn1.O=Cc1c[nH]c(-c2ccccc2F)c1>>Cn1cc(S(=O)(=O)n2cc(C=O)cc2-c2ccccc2F)cn1
FC1=C(C=CC=C1)C1=CC(=CN1)C=O.CN1N=CC(=C1)S(=O)(=O)Cl>>FC1=C(C=CC=C1)C1=CC(=CN1S(=O)(=O)C=1C=NN(C1)C)C=O
Cl[S:5]([c:4]1[cH:3][n:2]([CH3:1])[n:23][cH:22]1)(=[O:6])=[O:7].[nH:8]1[cH:9][c:10]([CH:11]=[O:12])[cH:13][c:14]1-[c:15]1[cH:16][cH:17][cH:18][cH:19][c:20]1[F:21]>>[CH3:1][n:2]1[cH:3][c:4]([S:5](=[O:6])(=[O:7])[n:8]2[cH:9][c:10]([CH:11]=[O:12])[cH:13][c:14]2-[c:15]2[cH:16][cH:17][cH:18][cH:19][c:20]2[F:21])[cH:22][n:23...
Cn1cc(S(=O)(=O)Cl)cn1.O=Cc1c[nH]c(-c2ccccc2F)c1
Cn1cc(S(=O)(=O)n2cc(C=O)cc2-c2ccccc2F)cn1
null
null
null
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cn[nH]c1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4]1:[c:5]:[#7;a:6]:[#7;a:7](-[C;D1;H3:8]):[c:9]:1.[O;D1;H0:10]=[C:11]-[c:12]1:[c:13]:[c:14](-[c:15]):[nH;D2;+0:16]:[c:17]:1>>[C;D1;H3:8]-[#7;a:7]1:[#7;a:6]:[c:5]:[c:4](-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[n;H0;D3;+0:16]2:[c:17]:[c:12](-[C:11]=[O;D1;H0:10]):[c:13]...
65
[{"value": 65.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
By a similar operation as in Reference Example 65 and using 5-(2-fluorophenyl)-1H-pyrrole-3-carbaldehyde (189 mg) and 1-methyl-1H-pyrazole-4-sulfonyl chloride (217 mg), the title compound was obtained as yellow crystals (yield 217 mg, 65%). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cn[nH]c1.c1cc[nH]c1.c1ccccc1
HCl
null
null
null
Cn1cc(S(=O)(=O)Cl)cn1.O=Cc1c[nH]c(-c2ccccc2F)c1>>Cn1cc(S(=O)(=O)n2cc(C=O)cc2-c2ccccc2F)cn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e5d0744914ac468f95ac2ef397a43598
Cc1ccccc1-c1cc(C=O)c[nH]1.O=S(=O)(Cl)c1cccnc1>>Cc1ccccc1-c1cc(C=O)cn1S(=O)(=O)c1cccnc1
CC1=C(C=CC=C1)C1=CC(=CN1)C=O.[H-].[Na+].C1COCCOCCOCCOCCO1.Cl.N1=CC(=CC=C1)S(=O)(=O)Cl>>CC1=C(C=CC=C1)C1=CC(=CN1S(=O)(=O)C=1C=NC=CC1)C=O
[CH3:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1-[c:8]1[cH:9][c:10]([CH:11]=[O:12])[cH:13][nH:14]1.Cl[S:15](=[O:16])(=[O:17])[c:18]1[cH:19][cH:20][cH:21][n:22][cH:23]1>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1-[c:8]1[cH:9][c:10]([CH:11]=[O:12])[cH:13][n:14]1[S:15](=[O:16])(=[O:17])[c:18]1[cH:19][cH:20][cH:21][n:22][cH:23...
Cc1ccccc1-c1cc(C=O)c[nH]1.O=S(=O)(Cl)c1cccnc1
Cc1ccccc1-c1cc(C=O)cn1S(=O)(=O)c1cccnc1
null
null
O1CCCC1.CN(C=O)C
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8].[O;D1;H0:9]=[C:10]-[c:11]1:[c:12]:[nH;D2;+0:13]:[c:14](-[c:15]):[c:16]:1>>[O;D1;H0:9]=[C:10]-[c:11]1:[c:12]:[n;H0;D3;+0:13](-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8]):[c:14](-[c:15]):[c:16]:1
80
[{"value": 80.0, "product": "CC1=C(C=CC=C1)C1=CC(=CN1S(=O)(=O)C=1C=NC=CC1)C=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 79.7, "product": "CC1=C(C=CC=C1)C1=CC(=CN1S(=O)(=O)C=1C=NC=CC1)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
5
MINUTE
To a solution of 5-(2-methylphenyl)-1H-pyrrole-3-carbaldehyde (371 mg) in tetrahydrofuran (10 mL) were added sodium hydride (60% in oil, 288 mg) and 15-crown-5 (1.32 g) at room temperature. After stirring for 5 min, a suspension of pyridine-3-sulfonyl chloride hydrochloride (642 mg) in N,N-dimethylformamide (5 mL) was ...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1ccccc1.c1cc[nH]c1.c1ccncc1
HCl
O1CCCC1.CN(C=O)C
null
0.083333
Cc1ccccc1-c1cc(C=O)c[nH]1.O=S(=O)(Cl)c1cccnc1>O1CCCC1.CN(C=O)C>Cc1ccccc1-c1cc(C=O)cn1S(=O)(=O)c1cccnc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-48d90f1e13ab4a4a9e015ba08e35838e
O=Cc1c[nH]c(-c2ccccc2F)c1Cl.O=S(=O)(Cl)c1cccnc1>>O=Cc1cn(S(=O)(=O)c2cccnc2)c(-c2ccccc2F)c1Cl
[H-].[Na+].ClC=1C(=CNC1C1=C(C=CC=C1)F)C=O.C1COCCOCCOCCOCCO1.Cl.N1=CC(=CC=C1)S(=O)(=O)Cl>>ClC=1C(=CN(C1C1=C(C=CC=C1)F)S(=O)(=O)C=1C=NC=CC1)C=O
[O:1]=[CH:2][c:3]1[cH:4][nH:5][c:15](-[c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[F:22])[c:23]1[Cl:24].Cl[S:6](=[O:7])(=[O:8])[c:9]1[cH:10][cH:11][cH:12][n:13][cH:14]1>>[O:1]=[CH:2][c:3]1[cH:4][n:5]([S:6](=[O:7])(=[O:8])[c:9]2[cH:10][cH:11][cH:12][n:13][cH:14]2)[c:15](-[c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[F:22])[c...
O=Cc1c[nH]c(-c2ccccc2F)c1Cl.O=S(=O)(Cl)c1cccnc1
O=Cc1cn(S(=O)(=O)c2cccnc2)c(-c2ccccc2F)c1Cl
null
null
O1CCCC1.O
Acylation
OtherReaction
b114dd962f9bbda43113428940d60131ff59184183aeb807b43d11ac89af2c38
97f7469015d28c17dd04331dd6d96add6c8052624259a8aad52811d647e364c7
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8].[O;D1;H0:9]=[C:10]-[c:11]1:[c:12]:[c:13](-[c:14]):[nH;D2;+0:15]:[c:16]:1>>[O;D1;H0:9]=[C:10]-[c:11]1:[c:12]:[c:13](-[c:14]):[n;H0;D3;+0:15](-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[#7;a:7]:[c:8]):[c:16]:1
78.5
[{"value": 78.0, "product": "ClC=1C(=CN(C1C1=C(C=CC=C1)F)S(=O)(=O)C=1C=NC=CC1)C=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 78.5, "product": "ClC=1C(=CN(C1C1=C(C=CC=C1)F)S(=O)(=O)C=1C=NC=CC1)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
15
MINUTE
A suspension of sodium hydride (60% in oil, 216 mg) in tetrahydrofuran (5 mL) was cooled to 0° C., a solution of 4-chloro-5-(2-fluorophenyl)-1H-pyrrole-3-carbaldehyde (335 mg) in tetrahydrofuran (5 mL), 15-crown-5 (991 mg), and pyridine-3-sulfonyl chloride hydrochloride (482 mg) were added at 10° C. or below. After sti...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1cc[nH]c1
c1cc[nH]c1
c1cc[nH]c1.c1ccncc1.c1ccccc1
HCl
O1CCCC1.O
0
0.25
O=Cc1c[nH]c(-c2ccccc2F)c1Cl.O=S(=O)(Cl)c1cccnc1>O1CCCC1.O>O=Cc1cn(S(=O)(=O)c2cccnc2)c(-c2ccccc2F)c1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-59a530d5cab849db9d60677d4cd7b986
O=C1CCC(=O)N1Cl.O=Cc1cc(-c2c(F)cccc2F)n(S(=O)(=O)c2cccnc2)c1>>O=Cc1cc(-c2c(F)cccc2F)n(S(=O)(=O)c2cccnc2)c1Cl
FC1=C(C(=CC=C1)F)C1=CC(=CN1S(=O)(=O)C=1C=NC=CC1)C=O.ClN1C(CCC1=O)=O.O>>ClC=1N(C(=CC1C=O)C1=C(C=CC=C1F)F)S(=O)(=O)C=1C=NC=CC1
O=C1CCC(=O)N1[Cl:25].[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[c:7]([F:8])[cH:9][cH:10][cH:11][c:12]2[F:13])[n:14]([S:15](=[O:16])(=[O:17])[c:18]2[cH:19][cH:20][cH:21][n:22][cH:23]2)[cH:24]1>>[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[c:7]([F:8])[cH:9][cH:10][cH:11][c:12]2[F:13])[n:14]([S:15](=[O:16])(=[O:17])[c:18]2[cH:19][cH:...
O=C1CCC(=O)N1Cl.O=Cc1cc(-c2c(F)cccc2F)n(S(=O)(=O)c2cccnc2)c1
O=Cc1cc(-c2c(F)cccc2F)n(S(=O)(=O)c2cccnc2)c1Cl
null
null
O1CCCC1.CN(C=O)C
Functional Group Interconversion
Chlorination
d90c51e04980e4fd5c41f2d9df1deefa5e01053fdb0009dabf82d5beacca27ac
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
O=C1-C-C-C(=O)-N-1-[Cl;H0;D1;+0:1].[#16:2]-[#7;a:3]1:[c:4]:[c:5]:[c:6](-[C:7]=[O;D1;H0:8]):[cH;D2;+0:9]:1>>[#16:2]-[#7;a:3]1:[c:4]:[c:5]:[c:6](-[C:7]=[O;D1;H0:8]):[c;H0;D3;+0:9]:1-[Cl;H0;D1;+0:1]
58.2
[{"value": 58.0, "product": "ClC=1N(C(=CC1C=O)C1=C(C=CC=C1F)F)S(=O)(=O)C=1C=NC=CC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 58.2, "product": "ClC=1N(C(=CC1C=O)C1=C(C=CC=C1F)F)S(=O)(=O)C=1C=NC=CC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
HOUR
To a solution of 5-(2,6-difluorophenyl)-1-(pyridin-3-ylsulfonyl)-1H-pyrrole-3-carbaldehyde (250 mg) in tetrahydrofuran (10 mL) and N,N-dimethylformamide (10 mL) was added N-chlorosuccinimide (1.06 g) and the mixture was stirred for 15 hr. Water was added to the reaction mixture, and the mixture was extracted with ethyl...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
C1CCNC1.c1cc[nH]c1
c1c[nH]cc1
c1c[nH]cc1.c1ccccc1.c1ccncc1
HO-
O1CCCC1.CN(C=O)C
null
15
O=C1CCC(=O)N1Cl.O=Cc1cc(-c2c(F)cccc2F)n(S(=O)(=O)c2cccnc2)c1>O1CCCC1.CN(C=O)C>O=Cc1cc(-c2c(F)cccc2F)n(S(=O)(=O)c2cccnc2)c1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-134dee9a914249bf8e51a4af82d15f95
O=C1CCC(=O)N1Cl.O=Cc1cc(-c2ccccc2F)n(S(=O)(=O)c2cccnc2)c1>>O=Cc1cc(-c2ccccc2F)n(S(=O)(=O)c2cccnc2)c1Cl
C(O)([O-])=O.[Na+].FC1=C(C=CC=C1)C1=CC(=CN1S(=O)(=O)C=1C=NC=CC1)C=O.ClN1C(CCC1=O)=O>>ClC=1N(C(=CC1C=O)C1=C(C=CC=C1)F)S(=O)(=O)C=1C=NC=CC1
O=C1CCC(=O)N1[Cl:24].[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][cH:9][cH:10][c:11]2[F:12])[n:13]([S:14](=[O:15])(=[O:16])[c:17]2[cH:18][cH:19][cH:20][n:21][cH:22]2)[cH:23]1>>[O:1]=[CH:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][cH:9][cH:10][c:11]2[F:12])[n:13]([S:14](=[O:15])(=[O:16])[c:17]2[cH:18][cH:19][cH:20][n:2...
O=C1CCC(=O)N1Cl.O=Cc1cc(-c2ccccc2F)n(S(=O)(=O)c2cccnc2)c1
O=Cc1cc(-c2ccccc2F)n(S(=O)(=O)c2cccnc2)c1Cl
null
null
CN(C=O)C
Functional Group Interconversion
Chlorination
d90c51e04980e4fd5c41f2d9df1deefa5e01053fdb0009dabf82d5beacca27ac
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=S(=O)(c1cccnc1)n1cccc1-c1ccccc1
O=C1-C-C-C(=O)-N-1-[Cl;H0;D1;+0:1].[#16:2]-[#7;a:3]1:[c:4]:[c:5]:[c:6](-[C:7]=[O;D1;H0:8]):[cH;D2;+0:9]:1>>[#16:2]-[#7;a:3]1:[c:4]:[c:5]:[c:6](-[C:7]=[O;D1;H0:8]):[c;H0;D3;+0:9]:1-[Cl;H0;D1;+0:1]
68.4
[{"value": 68.0, "product": "ClC=1N(C(=CC1C=O)C1=C(C=CC=C1)F)S(=O)(=O)C=1C=NC=CC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 68.4, "product": "ClC=1N(C(=CC1C=O)C1=C(C=CC=C1)F)S(=O)(=O)C=1C=NC=CC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
1
HOUR
To a solution of 5-(2-fluorophenyl)-1-(pyridin-3-ylsulfonyl)-1H-pyrrole-3-carbaldehyde (331 mg) in N,N-dimethylformamide (33 mL) was added N-chlorosuccinimide (268 mg) and the mixture was stirred at 60° C. for 1 hr. A saturated aqueous sodium hydrogencarbonate solution was added to the reaction mixture, and the mixture...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
C1CCNC1.c1cc[nH]c1
c1c[nH]cc1
c1c[nH]cc1.c1ccccc1.c1ccncc1
HO-
CN(C=O)C
60
1
O=C1CCC(=O)N1Cl.O=Cc1cc(-c2ccccc2F)n(S(=O)(=O)c2cccnc2)c1>CN(C=O)C>O=Cc1cc(-c2ccccc2F)n(S(=O)(=O)c2cccnc2)c1Cl