dataset_id
large_stringclasses
414 values
reaction_id
large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
reactant_smiles
large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-646e739121134fd1ac76394d8ef6bda5
C[Si](C)(C)c1c(F)cc(Cl)c(C=O)c1F.ClI>>O=Cc1c(Cl)cc(F)c(I)c1F
ClC1=CC(=C(C(=C1C=O)F)[Si](C)(C)C)F.ICl.ICl>>ClC1=CC(=C(C(=C1C=O)F)I)F
C[Si](C)(C)[c:9]1[c:7]([F:8])[cH:6][c:4]([Cl:5])[c:3]([CH:2]=[O:1])[c:11]1[F:12].Cl[I:10]>>[O:1]=[CH:2][c:3]1[c:4]([Cl:5])[cH:6][c:7]([F:8])[c:9]([I:10])[c:11]1[F:12]
C[Si](C)(C)c1c(F)cc(Cl)c(C=O)c1F.ClI
O=Cc1c(Cl)cc(F)c(I)c1F
null
null
C(Cl)Cl
Functional Group Interconversion
OtherReaction
047d69fb062d430b3c4234f4d9dc2362ad3d5bebae7ca0b8684377a133bdc02a
63283061f326a2fecd25d450c5b0c90ce007113b9f07907c978145ca0609298a
c1ccccc1
C-[Si](-C)(-C)-[c;H0;D3;+0:1](:[c:2](-[F;D1;H0:3]):[c:4]-[C:5]=[O;D1;H0:6]):[c:7](-[F;D1;H0:8]):[c:9].Cl-[I;H0;D1;+0:10]>>[F;D1;H0:3]-[c:2](:[c:4]-[C:5]=[O;D1;H0:6]):[c;H0;D3;+0:1](-[I;H0;D1;+0:10]):[c:7](-[F;D1;H0:8]):[c:9]
162.5
[{"value": 162.5, "product": "ClC1=CC(=C(C(=C1C=O)F)I)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
A solution of 6-chloro-2,4-difluoro-3-trimethylsilylbenzaldehyde (600 mg, 2.4 mmol) in methylene chloride (7 mL) was cooled to 0° C. and treated with solution of iodochloride (780 mg, 4.8 mmol) in methylene chloride (10 mL) and stirred at ambient temperature for 2 hours. Additional iodochloride (900 mg) was added and t...
10.6084/m9.figshare.5104873.v1
null
Silyl protective group
Aromatic halide
c1ccccc1
c1ccccc1
c1ccccc1
HCl
C(Cl)Cl
null
2
C[Si](C)(C)c1c(F)cc(Cl)c(C=O)c1F.ClI>C(Cl)Cl>O=Cc1c(Cl)cc(F)c(I)c1F
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c4361ce868eb4e1192e46ad2039e578f
CC(=O)OO.CI.Fc1cc(F)c(Br)cc1Br>>COc1cc(Br)c(F)cc1F
C(C)(=O)OO.C([O-])([O-])=O.[K+].[K+].IC.BrC1=CC(=C(C=C1F)F)Br.C(C)(C)[Mg]Cl.COB(OC)OC>>BrC1=C(C=C(C(=C1)OC)F)F
CC(=O)O[OH:2].I[CH3:1].Br[c:3]1[cH:4][c:5]([Br:6])[c:7]([F:8])[cH:9][c:10]1[F:11]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([Br:6])[c:7]([F:8])[cH:9][c:10]1[F:11]
CC(=O)OO.CI.Fc1cc(F)c(Br)cc1Br
COc1cc(Br)c(F)cc1F
null
null
C1CCOC1
Heteroatom Alkylation and Arylation
OtherReaction
35323bfc0b79a9b61c75d6aea2581c259b70e6e672b32672029e6a3625d5929f
c40ffbbc3249442e5ee39aaa69a55be7ac2fa45f48637395e415c565c1288454
c1ccccc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[F;D1;H0:5]):[c:6].C-C(=O)-O-[OH;D1;+0:7].I-[CH3;D1;+0:8]>>[CH3;D1;+0:8]-[O;H0;D2;+0:7]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[F;D1;H0:5]):[c:6]
23.2
[{"value": 23.2, "product": "BrC1=C(C=C(C(=C1)OC)F)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
30
MINUTE
To a solution of 1,3 dibromo-4,6-difluorobenzene (10.0 g, 37 mmol) in THF (50 mL) at −20° C. was added isopropyl magnesium chloride (2.0M in THF, 42 mmol) and the resulting solution warm to 0° C. and stirred for 30 minutes. Trimethylborate (4.7 g, 45 mmol) was added and the mixture stirred at ambient temperature for 1 ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Peroxide
Ether
c1ccccc1
c1ccccc1
c1ccccc1
HBr.I-
C1CCOC1
0
0.5
CC(=O)OO.CI.Fc1cc(F)c(Br)cc1Br>C1CCOC1>COc1cc(Br)c(F)cc1F
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9d5521e78560442b906e15943c2ba77c
COC(=O)c1nc(Cl)cc(NC(C)=O)c1Cl.COc1cc(B2OCCCO2)c(F)cc1Cl>>COC(=O)c1nc(-c2cc(OC)c(Cl)cc2F)cc(NC(C)=O)c1Cl
COC(=O)C1=NC(=CC(=C1Cl)NC(C)=O)Cl.ClC1=CC(=C(C=C1OC)B1OCCCO1)F.[F-].[Cs+].C1(=CC=CC=C1)P(CCCCP(C1=CC=CC=C1)C1=CC=CC=C1)C1=CC=CC=C1>>COC(=O)C1=NC(=CC(=C1Cl)NC(C)=O)C1=C(C=C(C(=C1)OC)Cl)F
Cl[c:7]1[n:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[c:24]([Cl:25])[c:19]([NH:20][C:21]([CH3:22])=[O:23])[cH:18]1.C1COB([c:8]2[cH:9][c:10]([O:11][CH3:12])[c:13]([Cl:14])[cH:15][c:16]2[F:17])OC1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[n:6][c:7](-[c:8]2[cH:9][c:10]([O:11][CH3:12])[c:13]([Cl:14])[cH:15][c:16]2[F:17])[cH:18][c:19]([NH:2...
COC(=O)c1nc(Cl)cc(NC(C)=O)c1Cl.COc1cc(B2OCCCO2)c(F)cc1Cl
COC(=O)c1nc(-c2cc(OC)c(Cl)cc2F)cc(NC(C)=O)c1Cl
null
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-]
O.C(C)#N
C-C Coupling
Suzuki coupling with boronic esters
24090aed37a48c66cce36a374df588b856a5a96d58744799fd5f32d2bb560bf0
48892094855745f5c51f8910c27ce7c101e08ad3f9da2a58d5512e3d9c1b432f
c1ccc(-c2ccccn2)cc1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]-[C:4](-[#8:5])=[O;D1;H0:6]):[c:7]:[c:8].[F;D1;H0:9]-[c:10](:[c:11]):[c;H0;D3;+0:12](-B1-O-C-C-C-O-1):[c:13]:[c:14]>>[#8:5]-[C:4](=[O;D1;H0:6])-[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:12](:[c:13]:[c:14]):[c:10](-[F;D1;H0:9]):[c:11]):[c:7]:[c:8]
75
[{"value": 75.0, "product": "COC(=O)C1=NC(=CC(=C1Cl)NC(C)=O)C1=C(C=C(C(=C1)OC)Cl)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 4-acetylamino-3,6-dichloropyridine carboxylic acid methyl ester (4.3 g, 0.016 mol), 2-(4-chloro-2-fluoro-5-methoxyphenyl)-[1,3,2]-dioxaborinane (4.5 g, 0.018 mol), cesium fluoride (3.5 g, 0.025 mol), and 1,4-bis(diphenylphosphino)butane (0.360 g, 0.0016 mol) in acetonitrile (100 mL) was degassed with nitr...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1ccncc1.B1OCCCO1.c1ccccc1
c1ccncc1.c1ccccc1
c1ccncc1.c1ccccc1
HCl.B
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].O.C(C)#N
null
null
COC(=O)c1nc(Cl)cc(NC(C)=O)c1Cl.COc1cc(B2OCCCO2)c(F)cc1Cl>C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].O.C(C)#N>COC(=O)c1nc(-c2cc(OC)c(Cl)cc2F)cc(NC(C)=O)c1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-100bc78c6db840f1b52b9e256a480b2c
COC(=O)c1n[c]([Sn]([CH3])([CH3])[CH3])cc(NC(C)=O)c1Cl.Cc1c(F)ccc(Br)c1F>>COC(=O)c1nc(-c2ccc(F)c(C)c2F)cc(NC(C)=O)c1Cl
BrC1=C(C(=C(C=C1)F)C)F.COC(=O)C1=NC(=CC(=C1Cl)NC(C)=O)[Sn](C)(C)C.C1(=CC=CC=C1)P(CCCCP(C1=CC=CC=C1)C1=CC=CC=C1)C1=CC=CC=C1.[F-].[Cs+]>>COC(=O)C1=NC(=CC(=C1Cl)NC(C)=O)C1=C(C(=C(C=C1)F)C)F
[CH3][Sn]([CH3])([CH3])[c:7]1[n:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[c:23]([Cl:24])[c:18]([NH:19][C:20]([CH3:21])=[O:22])[cH:17]1.Br[c:8]1[cH:9][cH:10][c:11]([F:12])[c:13]([CH3:14])[c:15]1[F:16]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[n:6][c:7](-[c:8]2[cH:9][cH:10][c:11]([F:12])[c:13]([CH3:14])[c:15]2[F:16])[cH:17][c:18]([NH:19...
COC(=O)c1n[c]([Sn]([CH3])([CH3])[CH3])cc(NC(C)=O)c1Cl.Cc1c(F)ccc(Br)c1F
COC(=O)c1nc(-c2ccc(F)c(C)c2F)cc(NC(C)=O)c1Cl
null
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-]
C(C)#N
C-C Coupling
Stille reaction_aryl
ce918bbb171f9e7bd99035931c043f0f33f636d165d8c0e73629d8717d6c595a
db27eeefac0475c6d74fa10b3167e95a61caaae74e8bbafd45892452c0c3d4d6
c1ccc(-c2ccccn2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[F;D1;H0:5]):[c:6].[#8:7]-[C:8](=[O;D1;H0:9])-[c:10]:[#7;a:11]:[c;H0;D3;+0:12](-[Sn](-[CH3])(-[CH3])-[CH3]):[c:13]:[c:14]>>[#8:7]-[C:8](=[O;D1;H0:9])-[c:10]:[#7;a:11]:[c;H0;D3;+0:12](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[F;D1;H0:5]):[c:6]):[c:13]:[c:14]
20
[{"value": 20.0, "product": "COC(=O)C1=NC(=CC(=C1Cl)NC(C)=O)C1=C(C(=C(C=C1)F)C)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 1-bromo-2,4-difluoro-3-methylbenzene (2.10 g, 0.09 mol), 4-acetylamino-3-chloro-6-trimethylstannylpyridine-2-carboxylic acid methyl ester (4.00 g, 0.01 mol), 1,4-bis(diphenylphosphino)butane (0.140 g, 0.0003 mol) and cesium fluoride (4.5 g, 0.03 mol) in acetonitrile (100 mL) was degassed with nitrogen. Pa...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Tin
null
c1ccncc1.c1ccccc1
c1ccncc1.c1ccccc1
c1ccncc1.c1ccccc1
HBr.Sn
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].C(C)#N
null
null
COC(=O)c1n[c]([Sn]([CH3])([CH3])[CH3])cc(NC(C)=O)c1Cl.Cc1c(F)ccc(Br)c1F>C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].C(C)#N>COC(=O)c1nc(-c2ccc(F)c(C)c2F)cc(NC(C)=O)c1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ef88bfceac19452d82b5de6467be35e3
COC(=O)c1nc(Cl)cc(NC(C)=O)c1Cl.COc1c(C(F)(F)F)cc[c]([Sn]([CH3])([CH3])[CH3])c1F>>COC(=O)c1nc(-c2ccc(C(F)(F)F)c(OC)c2F)cc(NC(C)=O)c1Cl
COC(=O)C1=NC(=CC(=C1Cl)NC(C)=O)Cl.FC1=C(C=CC(=C1OC)C(F)(F)F)[Sn](C)(C)C.[F-].[Cs+].C1(=CC=CC=C1)P(CCCCP(C1=CC=CC=C1)C1=CC=CC=C1)C1=CC=CC=C1>>COC(=O)C1=NC(=CC(=C1Cl)NC(C)=O)C1=C(C(=C(C=C1)C(F)(F)F)OC)F
Cl[c:7]1[n:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[c:27]([Cl:28])[c:22]([NH:23][C:24]([CH3:25])=[O:26])[cH:21]1.[CH3][Sn]([CH3])([CH3])[c:8]1[cH:9][cH:10][c:11]([C:12]([F:13])([F:14])[F:15])[c:16]([O:17][CH3:18])[c:19]1[F:20]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[n:6][c:7](-[c:8]2[cH:9][cH:10][c:11]([C:12]([F:13])([F:14])[F:15])...
COC(=O)c1nc(Cl)cc(NC(C)=O)c1Cl.COc1c(C(F)(F)F)cc[c]([Sn]([CH3])([CH3])[CH3])c1F
COC(=O)c1nc(-c2ccc(C(F)(F)F)c(OC)c2F)cc(NC(C)=O)c1Cl
null
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-]
C(C)#N
C-C Coupling
Stille reaction_aryl
ce918bbb171f9e7bd99035931c043f0f33f636d165d8c0e73629d8717d6c595a
db27eeefac0475c6d74fa10b3167e95a61caaae74e8bbafd45892452c0c3d4d6
c1ccc(-c2ccccn2)cc1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]-[C:4](-[#8:5])=[O;D1;H0:6]):[c:7]:[c:8].[CH3]-[Sn](-[CH3])(-[CH3])-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12](-[F;D1;H0:13]):[c:14]>>[#8:5]-[C:4](=[O;D1;H0:6])-[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12](-[F;D1;H0:13]):[c:14]):[c:7]:[c:8]
10
[{"value": 10.0, "product": "COC(=O)C1=NC(=CC(=C1Cl)NC(C)=O)C1=C(C(=C(C=C1)C(F)(F)F)OC)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In an oven dried, nitrogen flushed 100 mL 3 neck flask equipped with a condenser and a magnetic stirbar was dissolved methyl-4-acetamido-3,6-dichloropyridine-2-carboxylate (1.2 g, 4.6 mmol) and (2-fluoro-3-methoxy-4-trifluoromethylphenyl)trimethyl stannane (1.7 g, 4.6 mmol) in acetonitrile (15 mL) and the resulting sol...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Tin
null
c1ccncc1.c1ccccc1
c1ccncc1.c1ccccc1
c1ccncc1.c1ccccc1
HCl.Sn
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].C(C)#N
null
null
COC(=O)c1nc(Cl)cc(NC(C)=O)c1Cl.COc1c(C(F)(F)F)cc[c]([Sn]([CH3])([CH3])[CH3])c1F>C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].C(C)#N>COC(=O)c1nc(-c2ccc(C(F)(F)F)c(OC)c2F)cc(NC(C)=O)c1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-eeadaa8ae94740c897fe9c4f5f77ce63
COC(=O)c1nc(-c2ccc(Cl)cc2F)cc(N)c1Cl.O=[N+]([O-])[O-]>>COC(=O)c1nc(-c2cc([N+](=O)[O-])c(Cl)cc2F)cc(N)c1Cl
NC1=C(C(=NC(=C1)C1=C(C=C(C=C1)Cl)F)C(=O)OC)Cl.S(O)(O)(=O)=O.[N+](=O)([O-])[O-].[Na+]>>COC(=O)C1=NC(=CC(=C1Cl)N)C1=C(C=C(C(=C1)[N+](=O)[O-])Cl)F
[CH3:1][O:2][C:3](=[O:4])[c:5]1[n:6][c:7](-[c:8]2[cH:9][cH:10][c:14]([Cl:15])[cH:16][c:17]2[F:18])[cH:19][c:20]([NH2:21])[c:22]1[Cl:23].[O-][N+:11](=[O:12])[O-:13]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[n:6][c:7](-[c:8]2[cH:9][c:10]([N+:11](=[O:12])[O-:13])[c:14]([Cl:15])[cH:16][c:17]2[F:18])[cH:19][c:20]([NH2:21])[c:22]1[Cl...
COC(=O)c1nc(-c2ccc(Cl)cc2F)cc(N)c1Cl.O=[N+]([O-])[O-]
COC(=O)c1nc(-c2cc([N+](=O)[O-])c(Cl)cc2F)cc(N)c1Cl
null
null
null
Functional Group Addition
Aromatic nitration with NO3 salt
53848b8b2bb4e867226e49db2e60519b24be9379900e3ad7c56af54fe8fde7a5
ddce49825c02b8965f10c8d99e3c841d26e1f136da6037b417c09313e6d73097
c1ccc(-c2ccccn2)cc1
[Cl;D1;H0:1]-[c:2](:[c:3]):[cH;D2;+0:4]:[c:5]:[c:6].[O-]-[N+;H0;D3:7](-[O;-;D1;H0:8])=[O;D1;H0:9]>>[Cl;D1;H0:1]-[c:2](:[c:3]):[c;H0;D3;+0:4](-[N+;H0;D3:7](-[O;-;D1;H0:8])=[O;D1;H0:9]):[c:5]:[c:6]
84.4
[{"value": 84.4, "product": "COC(=O)C1=NC(=CC(=C1Cl)N)C1=C(C=C(C(=C1)[N+](=O)[O-])Cl)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
1.5
HOUR
Methyl 4-amino-3-chloro-6-(4-chloro-2-fluorophenyl)pyridine-2-carboxylate (1.0 g, 3.2 mmol) was added as a solid to well stirred concentrated sulfuric acid (16 mL) at 0° C. Sodium nitrate (0.29 g, 3.5 mmol) was added to the mixture and the resulting yellow solution was stirred at 0° C. for 1.5 hours then diluted with a...
10.6084/m9.figshare.5104873.v1
null
Nitrate
Nitro group
c1ccccc1
c1ccccc1
c1ccncc1.c1ccccc1
HO-
null
0
1.5
COC(=O)c1nc(-c2ccc(Cl)cc2F)cc(N)c1Cl.O=[N+]([O-])[O-]>>COC(=O)c1nc(-c2cc([N+](=O)[O-])c(Cl)cc2F)cc(N)c1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b5cfacbfd659408caba2c0154e739c11
COC(=O)c1nc(-c2cc([N+](=O)[O-])c(Cl)cc2F)cc(N)c1Cl>>COC(=O)c1nc(-c2cc(N)c(Cl)cc2F)cc(N)c1Cl
NC1=C(C(=NC(=C1)C1=C(C=C(C(=C1)[N+](=O)[O-])Cl)F)C(=O)OC)Cl>>COC(=O)C1=NC(=CC(=C1Cl)N)C1=C(C=C(C(=C1)N)Cl)F
O=[N+:11]([O-])[c:10]1[cH:9][c:8](-[c:7]2[n:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[c:20]([Cl:21])[c:18]([NH2:19])[cH:17]2)[c:15]([F:16])[cH:14][c:12]1[Cl:13]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[n:6][c:7](-[c:8]2[cH:9][c:10]([NH2:11])[c:12]([Cl:13])[cH:14][c:15]2[F:16])[cH:17][c:18]([NH2:19])[c:20]1[Cl:21]
COC(=O)c1nc(-c2cc([N+](=O)[O-])c(Cl)cc2F)cc(N)c1Cl
COC(=O)c1nc(-c2cc(N)c(Cl)cc2F)cc(N)c1Cl
null
[Fe]
C(C)(=O)O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc(-c2ccccn2)cc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
95.7
[{"value": 95.7, "product": "COC(=O)C1=NC(=CC(=C1Cl)N)C1=C(C=C(C(=C1)N)Cl)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
85
CELSIUS
null
null
Iron powder (0.78 g, 13.9 mmol) was added to a slurry of methyl 4-amino-3-chloro-6-(4-chloro-2-fluoro-5-nitrophenyl)pyridine-2-carboxylate (0.5 g, 1.39 mmol) in acetic acid (20 mL) in a 100 mL round bottomed flask. The mixture was heated to 85° C. for 15 minutes. then cooled to room temperature and filtered through cel...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccncc1.c1ccccc1
Other
[Fe].C(C)(=O)O
85
null
COC(=O)c1nc(-c2cc([N+](=O)[O-])c(Cl)cc2F)cc(N)c1Cl>[Fe].C(C)(=O)O>COC(=O)c1nc(-c2cc(N)c(Cl)cc2F)cc(N)c1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-934967c86b6e4b24b3451998f1aebc3d
COC(=O)c1nc(I)cc(NC(C)=O)c1Cl>>COC(=O)c1nc(I)cc(N)c1Cl
O.C(C)(=O)NC1=C(C(=NC(=C1)I)C(=O)OC)Cl.C(C)(=O)Cl>>NC1=C(C(=NC(=C1)I)C(=O)OC)Cl
CC(=O)[NH:11][c:10]1[cH:9][c:7]([I:8])[n:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[c:12]1[Cl:13]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[n:6][c:7]([I:8])[cH:9][c:10]([NH2:11])[c:12]1[Cl:13]
COC(=O)c1nc(I)cc(NC(C)=O)c1Cl
COC(=O)c1nc(I)cc(N)c1Cl
null
null
CO
Reduction
Hydrogenolysis of amides/imides/carbamates
755df58c254dea764fdda078ffd678ec540bba057c83683be04c253f1270ac7b
025f7cefe51e71668ad5d09fca32df168e9b538347403e4d5c1748073e538adc
c1ccncc1
C-C(=O)-[NH;D2;+0:1]-[c:2]1:[c:3]:[c:4]:[#7;a:5]:[c:6]:[c:7]:1>>[NH2;D1;+0:1]-[c:2]1:[c:3]:[c:4]:[#7;a:5]:[c:6]:[c:7]:1
78.6
[{"value": 78.6, "product": "NC1=C(C(=NC(=C1)I)C(=O)OC)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To solution of 4-acetylamino-3-chloro-6-iodopyridine-2-carboxylic acid, methyl ester (5.0 g, 14 mmol) in methanol (25 mL) was added acetyl chloride (1 mL) and the solution heated under reflux for 1 hour. The solution was cooled and water (25 mL) added and the precipitate was collected. Recrystallization from methanol g...
10.6084/m9.figshare.5104873.v1
null
Secondary amide
Primary amine
null
null
c1ccncc1
HO-
CO
null
null
COC(=O)c1nc(I)cc(NC(C)=O)c1Cl>CO>COC(=O)c1nc(I)cc(N)c1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ee79c5f4860c4f2f8025c67255b0b577
COC(=O)c1nc(I)cc(N)c1Cl.COc1c(Br)ccc(B(O)O)c1F>>COC(=O)c1nc(-c2ccc(Br)c(OC)c2F)cc(NC(C)=O)c1Cl
NC1=C(C(=NC(=C1)I)C(=O)OC)Cl.BrC1=C(C(=C(C=C1)B(O)O)F)OC.[F-].[Cs+].C(OC)COC>>C(C)(=O)NC1=C(C(=NC(=C1)C1=C(C(=C(C=C1)Br)OC)F)C(=O)OC)Cl
I[c:7]1[n:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[c:24]([Cl:25])[c:19]([NH2:20])[cH:18]1.OB([c:8]1[cH:9][cH:10][c:11]([Br:12])[c:13]([O:14][CH3:15])[c:16]1[F:17])[OH:23]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[n:6][c:7](-[c:8]2[cH:9][cH:10][c:11]([Br:12])[c:13]([O:14][CH3:15])[c:16]2[F:17])[cH:18][c:19]([NH:20][C:21]([CH3:22])=[O:...
COC(=O)c1nc(I)cc(N)c1Cl.COc1c(Br)ccc(B(O)O)c1F
COC(=O)c1nc(-c2ccc(Br)c(OC)c2F)cc(NC(C)=O)c1Cl
null
null
O
Acylation
OtherReaction
358e91ad2921a0b16e42cfb733731c0f0542fcb580c0e968be351aabcc6bc332
6ec000fb720526e36b2afdf13966b1f2a2c19b6625dec262e485ab5539e0008b
c1ccc(-c2ccccn2)cc1
I-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](-[C:4](-[#8:5])=[O;D1;H0:6]):[c:7]:[c:8](-[NH2;D1;+0:9]):[c:10]:1.O-B(-[OH;D1;+0:11])-[c;H0;D3;+0:12](:[c:13]:[c:14]):[c:15](-[F;D1;H0:16]):[c:17]>>[#8:5]-[C:4](=[O;D1;H0:6])-[c:3]1:[#7;a:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:12](:[c:13]:[c:14]):[c:15](-[F;D1;H0:16]):[c:17]):[c:10]:[c:8](-[NH;...
null
[]
85
CELSIUS
null
null
A solution of 4-amino-3-chloro-6-iodopyridine-2-carboxylic acid, methyl ester (1.1 g, 3.0 mmol), 4-bromo-2-fluoro-3-methoxyphenyl boronic acid (1.3 g, 4.5 mmol) and cesium fluoride (0.60 g, 4.0 mmole) in dimethoxyethane (2 mL) and water (2 mL) was de-aerated with a stream of nitrogen for 15 minutes before adding dichlo...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine.Boronic acid
Secondary amide
c1ccncc1.c1ccccc1
c1ccncc1.c1ccccc1
c1ccncc1.c1ccccc1
I-.B
O
85
null
COC(=O)c1nc(I)cc(N)c1Cl.COc1c(Br)ccc(B(O)O)c1F>O>COC(=O)c1nc(-c2ccc(Br)c(OC)c2F)cc(NC(C)=O)c1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b47ea4588ed34879940d3ad59339d2ce
CC(F)c1c(Cl)ccc(Br)c1Cl.COC(=O)c1n[c]([Sn]([CH3])([CH3])[CH3])cc(NC(C)=O)c1Cl>>COC(=O)c1nc(-c2ccc(Cl)c(C(C)F)c2Cl)cc(NC(C)=O)c1Cl
O.ClC1=C(C=CC(=C1C(C)F)Cl)Br.C(C)(=O)NC1=C(C(=NC(=C1)[Sn](C)(C)C)C(=O)OC)Cl.[F-].[Cs+]>>C(C)(=O)NC1=C(C(=NC(=C1)C1=C(C(=C(C=C1)Cl)C(C)F)Cl)C(=O)OC)Cl
Br[c:8]1[cH:9][cH:10][c:11]([Cl:12])[c:13]([CH:14]([CH3:15])[F:16])[c:17]1[Cl:18].[CH3][Sn]([CH3])([CH3])[c:7]1[n:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[c:25]([Cl:26])[c:20]([NH:21][C:22]([CH3:23])=[O:24])[cH:19]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[n:6][c:7](-[c:8]2[cH:9][cH:10][c:11]([Cl:12])[c:13]([CH:14]([CH3:15])[F:16])[...
CC(F)c1c(Cl)ccc(Br)c1Cl.COC(=O)c1n[c]([Sn]([CH3])([CH3])[CH3])cc(NC(C)=O)c1Cl
COC(=O)c1nc(-c2ccc(Cl)c(C(C)F)c2Cl)cc(NC(C)=O)c1Cl
null
[Cu](I)I.Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl
CN(C)C=O
C-C Coupling
Stille reaction_aryl
ce918bbb171f9e7bd99035931c043f0f33f636d165d8c0e73629d8717d6c595a
db27eeefac0475c6d74fa10b3167e95a61caaae74e8bbafd45892452c0c3d4d6
c1ccc(-c2ccccn2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[Cl;D1;H0:5]):[c:6].[#8:7]-[C:8](=[O;D1;H0:9])-[c:10]:[#7;a:11]:[c;H0;D3;+0:12](-[Sn](-[CH3])(-[CH3])-[CH3]):[c:13]:[c:14]>>[#8:7]-[C:8](=[O;D1;H0:9])-[c:10]:[#7;a:11]:[c;H0;D3;+0:12](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[Cl;D1;H0:5]):[c:6]):[c:13]:[c:14]
null
[]
null
null
null
null
A solution of 2,4 dichloro-3-(1-fluoroethyl)-bromobenzene (3.4 g, 12.5 mmol), 4-acetylamino-3-chloro-6-trimethylstannyl-pyridine-2-carboxylic acid, methyl ester (4.7 g, 12.5 mmol), copper iodide (0.4 g, 2.1 mmol), cesium fluoride (3.6 g, 25 mmol) and dichlorobis(triphenylphosphine)palladium (0.14 g, 2 mmol) in DMF (50 ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Tin
null
c1ccccc1.c1ccncc1
c1ccncc1.c1ccccc1
c1ccncc1.c1ccccc1
HBr.Sn
[Cu](I)I.Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.CN(C)C=O
null
null
CC(F)c1c(Cl)ccc(Br)c1Cl.COC(=O)c1n[c]([Sn]([CH3])([CH3])[CH3])cc(NC(C)=O)c1Cl>[Cu](I)I.Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.CN(C)C=O>COC(=O)c1nc(-c2ccc(Cl)c(C(C)F)c2Cl)cc(NC(C)=O)c1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9b6cfb7fb9434e5596bf36d9d9ffccdf
COC(=O)c1nc(Cl)cc(N)c1Cl.COc1c(C)ccc(B(O)O)c1F>>COC(=O)c1nc(-c2ccc(C)c(OC)c2F)cc(N)c1Cl
NC1=C(C(=NC(=C1)Cl)C(=O)OC)Cl.FC1=C(C=CC(=C1OC)C)B(O)O.[F-].[Cs+]>>NC1=C(C(=NC(=C1)C1=C(C(=C(C=C1)C)OC)F)C(=O)OC)Cl
Cl[c:7]1[n:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[c:21]([Cl:22])[c:19]([NH2:20])[cH:18]1.OB(O)[c:8]1[cH:9][cH:10][c:11]([CH3:12])[c:13]([O:14][CH3:15])[c:16]1[F:17]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[n:6][c:7](-[c:8]2[cH:9][cH:10][c:11]([CH3:12])[c:13]([O:14][CH3:15])[c:16]2[F:17])[cH:18][c:19]([NH2:20])[c:21]1[Cl:22]
COC(=O)c1nc(Cl)cc(N)c1Cl.COc1c(C)ccc(B(O)O)c1F
COC(=O)c1nc(-c2ccc(C)c(OC)c2F)cc(N)c1Cl
null
null
O.C(OC)COC
C-C Coupling
Suzuki coupling with boronic acids
07e9b6e71d806aa92d4573f3838e77c7c8344de3e5d5735ebdb5fc6862ebf27d
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccccn2)cc1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]-[C:4](-[#8:5])=[O;D1;H0:6]):[c:7]:[c:8].O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12](-[F;D1;H0:13]):[c:14]>>[#8:5]-[C:4](=[O;D1;H0:6])-[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12](-[F;D1;H0:13]):[c:14]):[c:7]:[c:8]
18.2
[{"value": 18.2, "product": "NC1=C(C(=NC(=C1)C1=C(C(=C(C=C1)C)OC)F)C(=O)OC)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
85
CELSIUS
null
null
A solution of 4-amino-3,6-dichloropyridine-2-carboxylic acid, methyl ester (0.24 g, 1.1 mmol), 2-fluoro-3-methoxy-4-methylphenyl boronic acid (0.30 g, 1.63 mmol) and cesium fluoride (3.0 g, 3.26 mmole) in dimethoxyethane (2 mL) and water (2 mL) was purged with a stream of nitrogen for 15 minutes before adding dichlorob...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccncc1.c1ccccc1
c1ccncc1.c1ccccc1
c1ccncc1.c1ccccc1
HCl.B
O.C(OC)COC
85
null
COC(=O)c1nc(Cl)cc(N)c1Cl.COc1c(C)ccc(B(O)O)c1F>O.C(OC)COC>COC(=O)c1nc(-c2ccc(C)c(OC)c2F)cc(N)c1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c6562d5666814b609b1d0aee0b8f25c4
CCOc1c(Cl)ccc(-c2cc(NC(C)=O)c(Cl)c(C(=O)OC)n2)c1F>>CCOc1c(Cl)ccc(-c2cc(N)c(Cl)c(C(=O)OC)n2)c1F
O.COC(=O)C1=NC(=CC(=C1Cl)NC(C)=O)C1=C(C(=C(C=C1)Cl)OCC)F.C(C)(=O)Cl>>COC(=O)C1=NC(=CC(=C1Cl)N)C1=C(C(=C(C=C1)Cl)OCC)F
CC(=O)[NH:13][c:12]1[cH:11][c:10](-[c:9]2[cH:8][cH:7][c:5]([Cl:6])[c:4]([O:3][CH2:2][CH3:1])[c:22]2[F:23])[n:21][c:16]([C:17](=[O:18])[O:19][CH3:20])[c:14]1[Cl:15]>>[CH3:1][CH2:2][O:3][c:4]1[c:5]([Cl:6])[cH:7][cH:8][c:9](-[c:10]2[cH:11][c:12]([NH2:13])[c:14]([Cl:15])[c:16]([C:17](=[O:18])[O:19][CH3:20])[n:21]2)[c:22]1[...
CCOc1c(Cl)ccc(-c2cc(NC(C)=O)c(Cl)c(C(=O)OC)n2)c1F
CCOc1c(Cl)ccc(-c2cc(N)c(Cl)c(C(=O)OC)n2)c1F
null
null
CO
Reduction
Hydrogenolysis of amides/imides/carbamates
755df58c254dea764fdda078ffd678ec540bba057c83683be04c253f1270ac7b
025f7cefe51e71668ad5d09fca32df168e9b538347403e4d5c1748073e538adc
c1ccc(-c2ccccn2)cc1
C-C(=O)-[NH;D2;+0:1]-[c:2]1:[c:3]:[c:4]:[#7;a:5]:[c:6]:[c:7]:1>>[NH2;D1;+0:1]-[c:2]1:[c:3]:[c:4]:[#7;a:5]:[c:6]:[c:7]:1
null
[]
null
null
null
null
To a solution of 4-acetylamino-3-chloro-6-(4-chloro-2-fluoro-3-ethoxyphenyl)pyridine-2-carboxylic acid methyl ester (0.5 g, 0.0013 mol) in methanol (10 mL) was added acetyl chloride (1 mL) and the solution heated under reflux for 1 hour. Water (2 mL) was added and resulting solid collected and dried to give 4-amino-3-c...
10.6084/m9.figshare.5104873.v1
null
Secondary amide
Primary amine
null
null
c1ccccc1.c1ccncc1
HO-
CO
null
null
CCOc1c(Cl)ccc(-c2cc(NC(C)=O)c(Cl)c(C(=O)OC)n2)c1F>CO>CCOc1c(Cl)ccc(-c2cc(N)c(Cl)c(C(=O)OC)n2)c1F
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a872daf99c7d4d28a236b7ecc55a65c9
CCO.COC(=O)c1nc(-c2ccc(Cl)c(OC)c2F)cc(N)c1Cl>>CCOC(=O)c1nc(-c2ccc(Cl)c(OC)c2F)cc(N)c1Cl
NC1=C(C(=NC(=C1)C1=C(C(=C(C=C1)Cl)OC)F)C(=O)OC)Cl.C(C)O>>NC1=C(C(=NC(=C1)C1=C(C(=C(C=C1)Cl)OC)F)C(=O)OCC)Cl
[CH3:1][CH2:2][OH:3].CO[C:4](=[O:5])[c:6]1[n:7][c:8](-[c:9]2[cH:10][cH:11][c:12]([Cl:13])[c:14]([O:15][CH3:16])[c:17]2[F:18])[cH:19][c:20]([NH2:21])[c:22]1[Cl:23]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[n:7][c:8](-[c:9]2[cH:10][cH:11][c:12]([Cl:13])[c:14]([O:15][CH3:16])[c:17]2[F:18])[cH:19][c:20]([NH2:21])[c:22]1[Cl:2...
CCO.COC(=O)c1nc(-c2ccc(Cl)c(OC)c2F)cc(N)c1Cl
CCOC(=O)c1nc(-c2ccc(Cl)c(OC)c2F)cc(N)c1Cl
null
CC([O-])C.CC([O-])C.CC([O-])C.CC([O-])C.[Ti+4]
null
Acylation
C-methylation
c42e047d71ad2593a6d29093d1fe2ca16ccfd6db7b15eecf1eab340181aef83e
cb08be6428b0a3737df44d00995165c06a05fb7dec4fab744c09315c4f7771d4
c1ccc(-c2ccccn2)cc1
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#7;a:5]:[c:6].[C;D1;H3:7]-[C:8]-[OH;D1;+0:9]>>[C;D1;H3:7]-[C:8]-[O;H0;D2;+0:9]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#7;a:5]:[c:6]
null
[]
null
null
null
null
To a solution of 4-amino-3-chloro-6-(4-chloro-2-fluoro-3-methoxyphenyl)pyridine-2-carboxylic acid, methyl ester (200 mg, 0.9 mmol) in ethanol (5 mL) was added a catalytic amount of titanium tetraisopropoxide and the solution heated under reflux for 2 hours. The solution was cooled and partitioned between ethyl acetate ...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary alcohol
Ester
null
null
c1ccncc1.c1ccccc1
HO-
CC([O-])C.CC([O-])C.CC([O-])C.CC([O-])C.[Ti+4]
null
null
CCO.COC(=O)c1nc(-c2ccc(Cl)c(OC)c2F)cc(N)c1Cl>CC([O-])C.CC([O-])C.CC([O-])C.CC([O-])C.[Ti+4]>CCOC(=O)c1nc(-c2ccc(Cl)c(OC)c2F)cc(N)c1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-17d8536a6d734624ab5d441efbf51b62
COc1c(C#N)cc(F)c(-c2cc(NC(C)=O)c(Cl)cn2)c1F.[OH-]>>COc1c(C#N)cc(F)c(-c2cc(N)c(Cl)c(C(=O)O)n2)c1F
Cl.C(C)(=O)NC1=C(C=NC(=C1)C1=C(C(=C(C=C1F)C#N)OC)F)Cl.[OH-].[Na+].CO>>NC1=C(C(=NC(=C1)C1=C(C(=C(C=C1F)C#N)OC)F)C(=O)O)Cl
C[C:18]([NH:14][c:13]1[cH:12][c:11](-[c:10]2[c:8]([F:9])[cH:7][c:4]([C:5]#[N:6])[c:3]([O:2][CH3:1])[c:22]2[F:23])[n:21][cH:17][c:15]1[Cl:16])=[O:19].[OH-:20]>>[CH3:1][O:2][c:3]1[c:4]([C:5]#[N:6])[cH:7][c:8]([F:9])[c:10](-[c:11]2[cH:12][c:13]([NH2:14])[c:15]([Cl:16])[c:17]([C:18](=[O:19])[OH:20])[n:21]2)[c:22]1[F:23]
COc1c(C#N)cc(F)c(-c2cc(NC(C)=O)c(Cl)cn2)c1F.[OH-]
COc1c(C#N)cc(F)c(-c2cc(N)c(Cl)c(C(=O)O)n2)c1F
null
null
O
Acylation
OtherReaction
a0000c18848ee93d6075d39c5138acbfb275189abc9fd6c7fafccbadcd149854
31b5c2cecdfb3a75e2cec361b135ff00b6a7e3073224bb1da24cc9c0c7780530
c1ccc(-c2ccccn2)cc1
C-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:3]-[c:4]1:[c:5]:[c:6]:[#7;a:7]:[cH;D2;+0:8]:[c:9]:1-[Cl;D1;H0:10].[OH-;D0:11]>>[Cl;D1;H0:10]-[c:9]1:[c:4](-[NH2;D1;+0:3]):[c:5]:[c:6]:[#7;a:7]:[c;H0;D3;+0:8]:1-[C;H0;D3;+0:1](=[O;D1;H0:2])-[OH;D1;+0:11]
null
[]
null
null
1
HOUR
A slurry of 4-acetylamino-3-chloro-6-(4-cyano-2,6-difluoro-3-methoxyphenyl)pyridine (0.13 g, 0.33 mmol) in methanol (5 mL) was treated with 1N sodium hydroxide (1.7 mL) and stirred at ambient temperature for 1 hour. The solution was diluted with water (15 mL) and acidified with 1N hydrochloric acid (1.7 mL) and the sol...
10.6084/m9.figshare.5104873.v1
null
Secondary amide
Carboxylic acid.Primary amine
c1ccncc1
c1ccncc1
c1ccccc1.c1ccncc1
Other
O
null
1
COc1c(C#N)cc(F)c(-c2cc(NC(C)=O)c(Cl)cn2)c1F.[OH-]>O>COc1c(C#N)cc(F)c(-c2cc(N)c(Cl)c(C(=O)O)n2)c1F
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6978c7a509c241098730825100bbf3f8
COc1c(C#N)cc(F)c(-c2cc(N)c(Cl)c(C(=O)O)n2)c1F.C[Si](C)(C)C=[N+]=[N-]>>COC(=O)c1nc(-c2c(F)cc(C#N)c(OC)c2F)cc(N)c1Cl
NC1=C(C(=NC(=C1)C1=C(C(=C(C=C1F)C#N)OC)F)C(=O)O)Cl.C[Si](C)(C)C=[N+]=[N-]>>NC1=C(C(=NC(=C1)C1=C(C(=C(C=C1F)C#N)OC)F)C(=O)OC)Cl
[OH:2][C:3](=[O:4])[c:5]1[n:6][c:7](-[c:8]2[c:9]([F:10])[cH:11][c:12]([C:13]#[N:14])[c:15]([O:16][CH3:17])[c:18]2[F:19])[cH:20][c:21]([NH2:22])[c:23]1[Cl:24].C[Si](C)(C)[CH:1]=[N+]=[N-]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[n:6][c:7](-[c:8]2[c:9]([F:10])[cH:11][c:12]([C:13]#[N:14])[c:15]([O:16][CH3:17])[c:18]2[F:19])[cH:20]...
COc1c(C#N)cc(F)c(-c2cc(N)c(Cl)c(C(=O)O)n2)c1F.C[Si](C)(C)C=[N+]=[N-]
COC(=O)c1nc(-c2c(F)cc(C#N)c(OC)c2F)cc(N)c1Cl
null
null
O1CCCC1.CO
Heteroatom Alkylation and Arylation
O-alkylation of carboxylic acids with diazo compounds
39589be0e9a30df66714fe618d22a8ac0fb24901dbf2ead1ab33e31556c7ac64
8b539baf7aeb5ab868833e33306bad77200a853d562904197e13de2e27e229d7
c1ccc(-c2ccccn2)cc1
C-[Si](-C)(-C)-[CH;D2;+0:1]=[N+]=[N-].[#7;a:2]:[c:3]-[C:4](=[O;D1;H0:5])-[OH;D1;+0:6]>>[#7;a:2]:[c:3]-[C:4](=[O;D1;H0:5])-[O;H0;D2;+0:6]-[CH3;D1;+0:1]
null
[]
null
null
null
null
A slurry of 4-amino-3-chloro-6-(4-cyano-2,6-difluoro-3-methoxyphenyl)pyridine-2-carboxlic acid in tetrahydrofuran (10 mL) and methanol (3 mL) was treated with trimethylsilyldiazomethane (0.64 g, 0.28 mL of a 2M solution in hexanes) at ambient temperature. After 1 hour the reaction mixture was quenched with acetic acid ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Diazo.Silyl protective group
Ester
null
null
c1ccncc1.c1ccccc1
Other
O1CCCC1.CO
null
null
COc1c(C#N)cc(F)c(-c2cc(N)c(Cl)c(C(=O)O)n2)c1F.C[Si](C)(C)C=[N+]=[N-]>O1CCCC1.CO>COC(=O)c1nc(-c2c(F)cc(C#N)c(OC)c2F)cc(N)c1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-93931ac2dfd44665925ad34be5a32c56
COC(=O)c1nc(-c2ccc(Cl)c(OCC(F)F)c2F)cc(N)c1Cl>>Nc1cc(-c2ccc(Cl)c(OCC(F)F)c2F)nc(C(=O)O)c1Cl
COC(=O)C1=NC(=CC(=C1Cl)N)C1=C(C(=C(C=C1)Cl)OCC(F)F)F.Cl>>NC1=C(C(=NC(=C1)C1=C(C(=C(C=C1)Cl)OCC(F)F)F)C(=O)O)Cl
C[O:22][C:20]([c:19]1[n:18][c:4](-[c:5]2[cH:6][cH:7][c:8]([Cl:9])[c:10]([O:11][CH2:12][CH:13]([F:14])[F:15])[c:16]2[F:17])[cH:3][c:2]([NH2:1])[c:23]1[Cl:24])=[O:21]>>[NH2:1][c:2]1[cH:3][c:4](-[c:5]2[cH:6][cH:7][c:8]([Cl:9])[c:10]([O:11][CH2:12][CH:13]([F:14])[F:15])[c:16]2[F:17])[n:18][c:19]([C:20](=[O:21])[OH:22])[c:2...
COC(=O)c1nc(-c2ccc(Cl)c(OCC(F)F)c2F)cc(N)c1Cl
Nc1cc(-c2ccc(Cl)c(OCC(F)F)c2F)nc(C(=O)O)c1Cl
null
null
CO.[OH-].[Na+]
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(-c2ccccn2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#7;a:5]>>[#7;a:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
87.5
[{"value": 87.5, "product": "NC1=C(C(=NC(=C1)C1=C(C(=C(C=C1)Cl)OCC(F)F)F)C(=O)O)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 4-amino-3-chloro-6-(4-chloro-2-fluoro-3-(2,2-difluoroethoxy)phenyl)pyridine-2-carboxylic acid methyl ester (0.300 g, 0.0008 mol) in methanol (5 mL) and sodium hydroxide (1N, 2 mL) was heated to reflux 1 hour and then acidified to pH 3 (concentrated hydrochloric acid) and allowed to cool. The resulting sol...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccncc1.c1ccccc1
Other
CO.[OH-].[Na+]
null
null
COC(=O)c1nc(-c2ccc(Cl)c(OCC(F)F)c2F)cc(N)c1Cl>CO.[OH-].[Na+]>Nc1cc(-c2ccc(Cl)c(OCC(F)F)c2F)nc(C(=O)O)c1Cl
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6668a3df1d294ec299f9a537d7d1fb2d
Brc1ccc(I)cc1.OB(O)c1cccc2c1oc1ccccc12>>Brc1ccc(-c2cccc3c2oc2ccccc23)cc1
C1=CC=C(C=2OC3=C(C21)C=CC=C3)B(O)O.BrC1=CC=C(C=C1)I.C([O-])([O-])=O.[Na+].[Na+]>>BrC1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1
I[c:5]1[cH:4][cH:3][c:2]([Br:1])[cH:20][cH:19]1.OB(O)[c:6]1[cH:7][cH:8][cH:9][c:10]2[c:11]1[o:12][c:13]1[cH:14][cH:15][cH:16][cH:17][c:18]21>>[Br:1][c:2]1[cH:3][cH:4][c:5](-[c:6]2[cH:7][cH:8][cH:9][c:10]3[c:11]2[o:12][c:13]2[cH:14][cH:15][cH:16][cH:17][c:18]32)[cH:19][cH:20]1
Brc1ccc(I)cc1.OB(O)c1cccc2c1oc1ccccc12
Brc1ccc(-c2cccc3c2oc2ccccc23)cc1
null
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1
C1(=CC=CC=C1)C.C(C)O
C-C Coupling
Suzuki coupling with boronic acids
a34fd3f8e97b635d120df300575865eab1505627afd99c75ec2034d5929796bd
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2cccc3c2oc2ccccc23)cc1
I-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9](:[c:10]):[#8;a:11]:[c:12]>>[c:10]:[c:9](:[#8;a:11]:[c:12]):[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:7]:[c:8]
null
[]
90
CELSIUS
null
null
A solution of dibenzofuran-4-boronic acid (1.0 g, 4.7 mmol) in ethanol (10 mL) was added to a stirred solution of 1-bromo-4-iodobenzene (1.33 g, 4.7 mmol) and tetrakis-(triphenylphosphine)-palladium(0) (271 mg, 5 mol %) in toluene (40 mL). 2 N sodium carbonate (4.7 mL, 9.4 mmol) was added and then the reaction was heat...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccc2c(c1)oc1ccccc12
c1ccccc1.c1ccc2c(c1)oc1ccccc12
c1ccccc1.c1ccc2c(c1)oc1ccccc12
HI.B
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)C.C(C)O
90
null
Brc1ccc(I)cc1.OB(O)c1cccc2c1oc1ccccc12>[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)C.C(C)O>Brc1ccc(-c2cccc3c2oc2ccccc23)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c107263d2030456a86346d5540e75258
Brc1ccc(-c2cccc3c2oc2ccccc23)cc1.O=Cc1ccc(B(O)O)cc1>>O=Cc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
C([O-])([O-])=O.[Na+].[Na+].C(=O)C1=CC=C(C=C1)B(O)O.BrC1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1>>C1=CC=C(C=2OC3=C(C21)C=CC=C3)C3=CC=C(C=C3)C3=CC=C(C=C3)C=O
Br[c:7]1[cH:8][cH:9][c:10](-[c:11]2[cH:12][cH:13][cH:14][c:15]3[c:16]2[o:17][c:18]2[cH:19][cH:20][cH:21][cH:22][c:23]32)[cH:24][cH:25]1.OB(O)[c:6]1[cH:5][cH:4][c:3]([CH:2]=[O:1])[cH:27][cH:26]1>>[O:1]=[CH:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10](-[c:11]3[cH:12][cH:13][cH:14][c:15]4[c:16]3[o:17][c:18]3[cH:19]...
Brc1ccc(-c2cccc3c2oc2ccccc23)cc1.O=Cc1ccc(B(O)O)cc1
O=Cc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
null
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1
C1(=CC=CC=C1)C.C(C)O
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:4]:[c:5]
null
[]
100
CELSIUS
null
null
A solution of 4-formylphenylboronic acid (0.9 g, 5.64 mmol) in ethanol (10 mL) was added to a stirred solution of the crude 4-(4-bromophenyl)-dibenzofuran (from the previous reaction) in toluene (40 mL). Tetrakis-(Triphenylphosphine)-palladium(0) (270 mg, 5 mol %) and 2 N sodium carbonate (4.7 mL, 9.4 mmol) were added ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1.c1ccc2c(c1)oc1ccccc12
HBr.B
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)C.C(C)O
100
null
Brc1ccc(-c2cccc3c2oc2ccccc23)cc1.O=Cc1ccc(B(O)O)cc1>[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)C.C(C)O>O=Cc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4b8c4540df4745e2b8c12305d363a39d
COC(=O)C(CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)OC(C)(C)C>>CC(C)(C)OC(=O)[C@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
[OH-].[Na+].COC(C(CSCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1)NC(=O)OC(C)(C)C)=O.CO.Cl>>C(C)(C)(C)OC(=O)[C@@H](C(=O)O)CSCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1
C[O:39][C:37]([CH:8](N[C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[CH2:9][S:10][CH2:11][c:12]1[cH:13][cH:14][c:15](-[c:16]2[cH:17][cH:18][c:19](-[c:20]3[cH:21][cH:22][cH:23][c:24]4[c:25]3[o:26][c:27]3[cH:28][cH:29][cH:30][cH:31][c:32]43)[cH:33][cH:34]2)[cH:35][cH:36]1)=[O:38]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C...
COC(=O)C(CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)OC(C)(C)C
CC(C)(C)OC(=O)[C@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
null
null
O1CCCC1.O
Miscellaneous
OtherReaction
4db8e1a49fb6f0bcc9ee9f32b36a5f4a173f45727a0b6ffb6ccaf6e3e1f4602b
67ba51d9ece8d51253e171fb304ba5fff35ed9a0dd60b78a97bb1cfca9faa562
c1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[CH;D3;+0:4](-N-[C;H0;D3;+0:5](=[O;D1;H0:6])-[#8:7]-[C:8](-[C;D1;H3:9])(-[C;D1;H3:10])-[C;D1;H3:11])-[C:12]-[#16:13]>>[#16:13]-[C:12]-[C@H;D3;+0:4](-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1])-[C;H0;D3;+0:5](=[O;D1;H0:6])-[#8:7]-[C:8](-[C;D1;H3:9])(-[C;D1;H3:10])-[C;D1;H3:11]
null
[]
null
null
null
null
2 N Sodium hydroxide solution (1.32 mL, 2.64 mmol) was added dropwise to a stirred solution of methyl-2-tert-butoxycarbonylamino-3-(4′-dibenzofuran-4-yl-biphenyl-4-ylmethylsulfanyl)propionate (500 mg, 0.88 mmol) in tetrahydrofuran (15 mL) and methanol (3 mL). The clear reaction mixture was stirred at room temperature u...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ester
Carboxylic acid.Ester
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)oc1ccccc12
Other
O1CCCC1.O
null
null
COC(=O)C(CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)OC(C)(C)C>O1CCCC1.O>CC(C)(C)OC(=O)[C@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5c2207eb52b04a02af89969c315ff374
COC(=O)C(CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)OC(C)(C)C>>COC(=O)C(N)CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
C([O-])(O)=O.[Na+].[Si](C)(C)(C)I.COC(C(CSCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1)NC(=O)OC(C)(C)C)=O.C(Cl)Cl>>COC(C(CSCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1)N)=O
CC(C)(C)OC(=O)[NH:6][CH:5]([C:3]([O:2][CH3:1])=[O:4])[CH2:7][S:8][CH2:9][c:10]1[cH:11][cH:12][c:13](-[c:14]2[cH:15][cH:16][c:17](-[c:18]3[cH:19][cH:20][cH:21][c:22]4[c:23]3[o:24][c:25]3[cH:26][cH:27][cH:28][cH:29][c:30]43)[cH:31][cH:32]2)[cH:33][cH:34]1>>[CH3:1][O:2][C:3](=[O:4])[CH:5]([NH2:6])[CH2:7][S:8][CH2:9][c:10]...
COC(=O)C(CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)OC(C)(C)C
COC(=O)C(N)CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
null
null
O
Reduction
Hydrogenolysis of amides/imides/carbamates
3c33dd2a2d355ee5ba0287367e209aa147a39aa00607f0c95fb2bf1ade45d014
c5b5dffe7dd8beebdc1baa8b5b05300a9f7079e65dcfd42ade6f8a77ff09537d
c1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[C:2](-[C:3])-[C:4](=[O;D1;H0:5])-[#8:6]-[C;D1;H3:7]>>[C:3]-[C:2](-[NH2;D1;+0:1])-[C:4](=[O;D1;H0:5])-[#8:6]-[C;D1;H3:7]
null
[]
null
null
25
MINUTE
TMS-I (290 mg, 0.21 mL, 1.45 mmol) was added dropwise to a stirred solution of methyl-2-tert-butoxycarbonylamino-3-(4′-dibenzofuran-4-yl-biphenyl-4-ylmethyl-sulfanyl)-propionate (748 mg, 1.32 mmol) in anhyd methylene chloride (20 mL). The reaction mixture was stirred at room temperature for 20-30 min (TLC control), and...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Primary amine
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)oc1ccccc12
HO-
O
null
0.416667
COC(=O)C(CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)OC(C)(C)C>O>COC(=O)C(N)CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5642754eba5c41788b001474b44a80fb
COC(=O)C(N)CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1.O=C(O)c1cc(C(F)(F)F)ccc1F>>COC(=O)C(CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)c1cc(C(F)(F)F)ccc1F
FC1=C(C(=O)O)C=C(C=C1)C(F)(F)F.COC(C(CSCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1)N)=O.CCN=C=NCCCN(C)C.C(C)N(CC)CC>>COC(C(CSCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1)NC(C1=C(C=CC(=C1)C(F)(F)F)F)=O)=O
[CH3:1][O:2][C:3](=[O:4])[CH:5]([CH2:6][S:7][CH2:8][c:9]1[cH:10][cH:11][c:12](-[c:13]2[cH:14][cH:15][c:16](-[c:17]3[cH:18][cH:19][cH:20][c:21]4[c:22]3[o:23][c:24]3[cH:25][cH:26][cH:27][cH:28][c:29]43)[cH:30][cH:31]2)[cH:32][cH:33]1)[NH2:34].O[C:35](=[O:36])[c:37]1[cH:38][c:39]([C:40]([F:41])([F:42])[F:43])[cH:44][cH:45...
COC(=O)C(N)CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1.O=C(O)c1cc(C(F)(F)F)ccc1F
COC(=O)C(CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)c1cc(C(F)(F)F)ccc1F
null
null
O.C(Cl)Cl
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(NCCSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C:6]-[C:7](-[NH2;D1;+0:8])-[C:9](=[O;D1;H0:10])-[#8:11]-[C;D1;H3:12]>>[C:6]-[C:7](-[NH;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5])-[C:9](=[O;D1;H0:10])-[#8:11]-[C;D1;H3:12]
null
[]
null
null
5
HOUR
2-Fluoro-5-trifluoromethylbenzoic acid (49 mg, 0.24 mmol) was added to a stirred solution of methyl-2-amino-3-(4′-dibenzofuran-4-ylbipheny-4-ylmethylsulfanyl)-propionate (92 mg, 0.2 mmol), EDCI (58 mg, 0.3 mmol) and triethylamine (404 mg, 0.56 mL, 0.4 mmol) in anhyd methylene chloride (5 mL). The reaction mixture was s...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)oc1ccccc12.c1ccccc1
HO-
O.C(Cl)Cl
null
5
COC(=O)C(N)CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1.O=C(O)c1cc(C(F)(F)F)ccc1F>O.C(Cl)Cl>COC(=O)C(CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)c1cc(C(F)(F)F)ccc1F
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0661e5a39dd14691ab85ae8c07e99e14
COC(=O)C(CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)c1cc(C(F)(F)F)ccc1F>>O=C(NC(CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O)c1cc(C(F)(F)F)ccc1F
[OH-].[Na+].COC(C(CSCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1)NC(C1=C(C=CC(=C1)C(F)(F)F)F)=O)=O.Cl>>C1=CC=C(C=2OC3=C(C21)C=CC=C3)C3=CC=C(C2=CC=C(C=C2)CSCC(C(=O)O)NC(C2=C(C=CC(=C2)C(F)(F)F)F)=O)C=C3
C[O:35][C:33]([CH:4]([NH:3][C:2](=[O:1])[c:36]1[cH:37][c:38]([C:39]([F:40])([F:41])[F:42])[cH:43][cH:44][c:45]1[F:46])[CH2:5][S:6][CH2:7][c:8]1[cH:9][cH:10][c:11](-[c:12]2[cH:13][cH:14][c:15](-[c:16]3[cH:17][cH:18][cH:19][c:20]4[c:21]3[o:22][c:23]3[cH:24][cH:25][cH:26][cH:27][c:28]43)[cH:29][cH:30]2)[cH:31][cH:32]1)=[O...
COC(=O)C(CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)c1cc(C(F)(F)F)ccc1F
O=C(NC(CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O)c1cc(C(F)(F)F)ccc1F
null
null
O1CCCC1.O.CO
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C(NCCSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)c1ccccc1
C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
null
[]
null
null
null
null
2 N Sodium hydroxide solution (0.25 mL, 0.5 mmol) was added dropwise to a stirred solution of methyl-3-(4′-dibenzofuran-4-yl-biphen-4ylmethylsulfanyl)-2(2-fluoro-5-trifluoromethylbenzoylamino)-propionate (110 mg, 0.17 mmol) in tetrahydrofuran (5 mL) and methanol (1 mL). The clear reaction mixture was stirred at room te...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)oc1ccccc12.c1ccccc1
Other
O1CCCC1.O.CO
null
null
COC(=O)C(CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)c1cc(C(F)(F)F)ccc1F>O1CCCC1.O.CO>O=C(NC(CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O)c1cc(C(F)(F)F)ccc1F
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-113365e68b154ac1a705d59bf018c6dc
CC(C)(C)OC(=O)N[C@@](C)(CSCc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)[O-]>>CC(C)(C)OC(=O)N[C@@H](CSCc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)O
[OH-].[Na+].C[C@@](C(=O)[O-])(CSCC1=CC=C(C=C1)C1=CC=C(C=C1)N1C=CC2=CC=CC=C12)NC(=O)OC(C)(C)C.Cl>>C(C)(C)(C)OC(=O)N[C@H](C(=O)O)CSCC1=CC=C(C=C1)C1=CC=C(C=C1)N1C=CC2=CC=CC=C12
C[C@:9]([NH:8][C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])([CH2:10][S:11][CH2:12][c:13]1[cH:14][cH:15][c:16](-[c:17]2[cH:18][cH:19][c:20](-[n:21]3[cH:22][cH:23][c:24]4[cH:25][cH:26][cH:27][cH:28][c:29]34)[cH:30][cH:31]2)[cH:32][cH:33]1)[C:34](=[O:35])[O-:36]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[NH:8][...
CC(C)(C)OC(=O)N[C@@](C)(CSCc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)[O-]
CC(C)(C)OC(=O)N[C@@H](CSCc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)O
null
null
O1CCCC1.O.CO
Miscellaneous
OtherReaction
a6b8ab131e7f70f6daa606d152ad1c80317c30ce07f436c723a799e222d8098f
d003579d88c8e6390ed4fac608b8ce68d334559ff02e2f3d9c9936750b60a874
c1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1
C-[C@;H0;D4;+0:1](-[#7:2]-[C:3](=[O;D1;H0:4])-[#8:5]-[C:6](-[C;D1;H3:7])(-[C;D1;H3:8])-[C;D1;H3:9])(-[C:10]-[#16:11])-[C:12](-[O-;H0;D1:13])=[O;D1;H0:14]>>[#16:11]-[C:10]-[C@H;D3;+0:1](-[#7:2]-[C:3](=[O;D1;H0:4])-[#8:5]-[C:6](-[C;D1;H3:7])(-[C;D1;H3:8])-[C;D1;H3:9])-[C:12](=[O;D1;H0:14])-[OH;D1;+0:13]
null
[]
null
null
null
null
1N Sodium hydroxide solution (2.14 mL, 2.14 mmol) was added dropwise to a stirred solution of (2R)-Methyl-tert-butoxycarbonylamino-3-(4′-indol-1-ylbiphen-4-ylmethylsulfanyl)-propionate (552 mg, 1.07 mmol) in tetrahydrofuran (15 mL) and methanol (3 mL). The clear reaction mixture was stirred at room temperature until th...
10.6084/m9.figshare.5104873.v1
null
null
Carboxylic acid
null
null
c1ccccc1.c1ccccc1.c1ccc2[nH]ccc2c1
Other
O1CCCC1.O.CO
null
null
CC(C)(C)OC(=O)N[C@@](C)(CSCc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)[O-]>O1CCCC1.O.CO>CC(C)(C)OC(=O)N[C@@H](CSCc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3c6a5b69c8124acf806461d03a805065
CC(C)(C)OC(=O)N[C@@H](CSCc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)O>>CC(C)(C)OC(=O)N[C@@H](CS(=O)Cc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)O
B1(OO1)[O-].O.O.O.O.[Na+].C(C)(C)(C)OC(=O)N[C@H](C(=O)O)CSCC1=CC=C(C=C1)C1=CC=C(C=C1)N1C=CC2=CC=CC=C12>>C(C)(C)(C)OC(=O)N[C@H](C(=O)O)CS(=O)CC1=CC=C(C=C1)C1=CC=C(C=C1)N1C=CC2=CC=CC=C12
[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[NH:8][C@@H:9]([CH2:10][S:11][CH2:13][c:14]1[cH:15][cH:16][c:17](-[c:18]2[cH:19][cH:20][c:21](-[n:22]3[cH:23][cH:24][c:25]4[cH:26][cH:27][cH:28][cH:29][c:30]34)[cH:31][cH:32]2)[cH:33][cH:34]1)[C:35](=[O:36])[OH:37]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[NH:8][C...
CC(C)(C)OC(=O)N[C@@H](CSCc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)O
CC(C)(C)OC(=O)N[C@@H](CS(=O)Cc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)O
null
null
C(C)(=O)O.C(C)(=O)OCC
Oxidation
Sulfanyl to sulfinyl
9edfaf6d72a81452ea8e3a1cdcb10a58409fff36608e97019e7273998b3d5373
f5f6bb6ca76a2267cd589767b4d67e7a17ab1ac383eeb6143dcd5d92e00e1b6a
c1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1
[O;D1;H0:1]=[C:2](-[O;D1;H1:3])-[C:4]-[C:5]-[S;H0;D2;+0:6]-[C:7]-[c:8]>>[O;D1;H0:9]=[S;H0;D3;+0:6](-[C:5]-[C:4]-[C:2](=[O;D1;H0:1])-[O;D1;H1:3])-[C:7]-[c:8]
null
[]
40
CELSIUS
2
HOUR
Sodium perborate tetrahydrate (151 mg, 0.95 mmol) was added as a solid to a stirred solution of (2R)-tert-Butoxycarbonylamino-3-(4′-indol-1-ylbiphen-4-ylmethylsulfanyl)-propionic acid (380 mg, 0.76 mmol) in acetic acid (10 mL) at 40° C. This solution was stirred at 40° C. for 2 hours (HPLC control) and then diluted wit...
10.6084/m9.figshare.5104873.v1
null
Monosulfide
Sulfoxide
null
null
c1ccccc1.c1ccccc1.c1ccc2[nH]ccc2c1
null
C(C)(=O)O.C(C)(=O)OCC
40
2
CC(C)(C)OC(=O)N[C@@H](CSCc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)O>C(C)(=O)O.C(C)(=O)OCC>CC(C)(C)OC(=O)N[C@@H](CS(=O)Cc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b6d87d33e4204defae757acd759b3761
CC(C)(C)OC(=O)N[C@@](C)(CSCc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)[O-]>>COC(=O)[C@@H](N)CSCc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1
[Si](C)(C)(C)I.C[C@@](C(=O)[O-])(CSCC1=CC=C(C=C1)C1=CC=C(C=C1)N1C=CC2=CC=CC=C12)NC(=O)OC(C)(C)C.C([O-])(O)=O.[Na+]>>COC([C@H](CSCC1=CC=C(C=C1)C1=CC=C(C=C1)N1C=CC2=CC=CC=C12)N)=O
CC(C)(C)OC(=O)[NH:6][C@:5](C)([C:3]([O-:2])=[O:4])[CH2:7][S:8][CH2:9][c:10]1[cH:11][cH:12][c:13](-[c:14]2[cH:15][cH:16][c:17](-[n:18]3[cH:19][cH:20][c:21]4[cH:22][cH:23][cH:24][cH:25][c:26]34)[cH:27][cH:28]2)[cH:29][cH:30]1>>[CH3:1][O:2][C:3](=[O:4])[C@@H:5]([NH2:6])[CH2:7][S:8][CH2:9][c:10]1[cH:11][cH:12][c:13](-[c:14...
CC(C)(C)OC(=O)N[C@@](C)(CSCc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)[O-]
COC(=O)[C@@H](N)CSCc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1
null
null
C(Cl)Cl
Miscellaneous
OtherReaction
47e29fef19aa31584b7fe52e994859163ada510d2b35acbed20cc1771c93a6f0
59f513d0431a3c0eec75fc6904881dfd8f6bfaabbb8014f6d2acaff8b29e8c08
c1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[C@@;H0;D4;+0:2](-C)(-[C:3]-[#16:4])-[C:5](-[O-;H0;D1:6])=[O;D1;H0:7]>>[#16:4]-[C:3]-[C@H;D3;+0:2](-[NH2;D1;+0:1])-[C:5](=[O;D1;H0:7])-[O;H0;D2;+0:6]-[C;D1;H3:8]
95
[{"value": 95.0, "product": "COC([C@H](CSCC1=CC=C(C=C1)C1=CC=C(C=C1)N1C=CC2=CC=CC=C12)N)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
10
MINUTE
TMSI (1.56 mL, 10.63 mmol) was added dropwise to a stirred solution of (2R)-methyl-tert-butoxycarbonylamino-3-(4′-indol-1-ylbiphen-4-ylmethylsulfanyl)-propionate (4.47 g, 8.66 mmol) in anhydrous methylene chloride (50 mL). The reaction was stirred for 10 mins. and then poured into 1N sodium bicarbonate solution (50 mL)...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Ester.Primary amine
null
null
c1ccccc1.c1ccccc1.c1ccc2[nH]ccc2c1
HO-
C(Cl)Cl
null
0.166667
CC(C)(C)OC(=O)N[C@@](C)(CSCc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)[O-]>C(Cl)Cl>COC(=O)[C@@H](N)CSCc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4f12f4d1314d41ae89b3304c88990bfc
O=C(Cc1cccc([N+](=O)[O-])c1)N[C@@H](CSCc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)O>>O=C(Cc1cccc([N+](=O)[O-])c1)N[C@@H](CS(=O)Cc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)O
B1(OO1)[O-].O.O.O.O.[Na+].N1(C=CC2=CC=CC=C12)C1=CC=C(C2=CC=C(C=C2)CSC[C@@H](C(=O)O)NC(CC2=CC(=CC=C2)[N+](=O)[O-])=O)C=C1>>N1(C=CC2=CC=CC=C12)C1=CC=C(C2=CC=C(C=C2)CS(=O)C[C@@H](C(=O)O)NC(CC2=CC(=CC=C2)[N+](=O)[O-])=O)C=C1
[O:1]=[C:2]([CH2:3][c:4]1[cH:5][cH:6][cH:7][c:8]([N+:9](=[O:10])[O-:11])[cH:12]1)[NH:13][C@@H:14]([CH2:15][S:16][CH2:18][c:19]1[cH:20][cH:21][c:22](-[c:23]2[cH:24][cH:25][c:26](-[n:27]3[cH:28][cH:29][c:30]4[cH:31][cH:32][cH:33][cH:34][c:35]34)[cH:36][cH:37]2)[cH:38][cH:39]1)[C:40](=[O:41])[OH:42]>>[O:1]=[C:2]([CH2:3][c...
O=C(Cc1cccc([N+](=O)[O-])c1)N[C@@H](CSCc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)O
O=C(Cc1cccc([N+](=O)[O-])c1)N[C@@H](CS(=O)Cc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)O
null
null
C(C)(=O)O.C(C)(=O)OCC
Oxidation
Sulfanyl to sulfinyl
9edfaf6d72a81452ea8e3a1cdcb10a58409fff36608e97019e7273998b3d5373
f5f6bb6ca76a2267cd589767b4d67e7a17ab1ac383eeb6143dcd5d92e00e1b6a
O=C(Cc1ccccc1)NCCS(=O)Cc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1
[O;D1;H0:1]=[C:2](-[O;D1;H1:3])-[C:4]-[C:5]-[S;H0;D2;+0:6]-[C:7]-[c:8]>>[O;D1;H0:9]=[S;H0;D3;+0:6](-[C:5]-[C:4]-[C:2](=[O;D1;H0:1])-[O;D1;H1:3])-[C:7]-[c:8]
61.1
[{"value": 61.0, "product": "N1(C=CC2=CC=CC=C12)C1=CC=C(C2=CC=C(C=C2)CS(=O)C[C@@H](C(=O)O)NC(CC2=CC(=CC=C2)[N+](=O)[O-])=O)C=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 61.1, "product": "N1(C=CC2=CC=CC=C12)C1=CC=C(C2=CC=C(C=C2)CS(=O)C[C@@H](C(=O)O)NC(CC2=CC(=CC=C2)[N+](=O)[O-])=O)C=C1", "details": "...
40
CELSIUS
2
HOUR
Sodium perborate tetrahydrate (97 mg, 0.63 mmol) was added as a solid to a stirred solution of (2R)-3-(4′-Indol-1-ylbiphen-4-ylmethylsulfanyl)-2-[2-(3-nitrophenyl)-acetylamino]-propionic acid (330 mg, 0.58 mmol) in acetic acid (10 mL) at 40° C. This solution was stirred at 40° C. for 2 hours (HPLC control) and then dil...
10.6084/m9.figshare.5104873.v1
null
Monosulfide
Sulfoxide
null
null
c1ccccc1.c1ccccc1.c1ccccc1.c1ccc2[nH]ccc2c1
null
C(C)(=O)O.C(C)(=O)OCC
40
2
O=C(Cc1cccc([N+](=O)[O-])c1)N[C@@H](CSCc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)O>C(C)(=O)O.C(C)(=O)OCC>O=C(Cc1cccc([N+](=O)[O-])c1)N[C@@H](CS(=O)Cc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9c736471cd2749cb9d11c5a8a992e28d
O=C(Cc1ccccc1)N[C@@H](CSCc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)O>>O=C(Cc1ccccc1)N[C@@H](CS(=O)Cc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)O
B1(OO1)[O-].O.O.O.O.[Na+].N1(C=CC2=CC=CC=C12)C1=CC=C(C2=CC=C(C=C2)CSC[C@@H](C(=O)O)NC(CC2=CC=CC=C2)=O)C=C1>>N1(C=CC2=CC=CC=C12)C1=CC=C(C2=CC=C(C=C2)CS(=O)C[C@@H](C(=O)O)NC(CC2=CC=CC=C2)=O)C=C1
[O:1]=[C:2]([CH2:3][c:4]1[cH:5][cH:6][cH:7][cH:8][cH:9]1)[NH:10][C@@H:11]([CH2:12][S:13][CH2:15][c:16]1[cH:17][cH:18][c:19](-[c:20]2[cH:21][cH:22][c:23](-[n:24]3[cH:25][cH:26][c:27]4[cH:28][cH:29][cH:30][cH:31][c:32]34)[cH:33][cH:34]2)[cH:35][cH:36]1)[C:37](=[O:38])[OH:39]>>[O:1]=[C:2]([CH2:3][c:4]1[cH:5][cH:6][cH:7][c...
O=C(Cc1ccccc1)N[C@@H](CSCc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)O
O=C(Cc1ccccc1)N[C@@H](CS(=O)Cc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)O
null
null
C(C)(=O)O.C(C)(=O)OCC
Oxidation
Sulfanyl to sulfinyl
9edfaf6d72a81452ea8e3a1cdcb10a58409fff36608e97019e7273998b3d5373
f5f6bb6ca76a2267cd589767b4d67e7a17ab1ac383eeb6143dcd5d92e00e1b6a
O=C(Cc1ccccc1)NCCS(=O)Cc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1
[O;D1;H0:1]=[C:2](-[O;D1;H1:3])-[C:4]-[C:5]-[S;H0;D2;+0:6]-[C:7]-[c:8]>>[O;D1;H0:9]=[S;H0;D3;+0:6](-[C:5]-[C:4]-[C:2](=[O;D1;H0:1])-[O;D1;H1:3])-[C:7]-[c:8]
null
[]
40
CELSIUS
2
HOUR
Sodium perborate tetrahydrate (97 mg, 0.63 mmol) was added as a solid to a stirred solution of (2R)-3-(4′-indol-1-ylbiphen-4-ylmethylsulfanyl)-2-phenylacetylamino-propionic acid (300 mg, 0.58 mmol) in acetic acid (10 mL) at 40° C. This solution was stirred at 40° C. for 2 hours (HPLC control) and then diluted with ethy...
10.6084/m9.figshare.5104873.v1
null
Monosulfide
Sulfoxide
null
null
c1ccccc1.c1ccccc1.c1ccccc1.c1ccc2[nH]ccc2c1
null
C(C)(=O)O.C(C)(=O)OCC
40
2
O=C(Cc1ccccc1)N[C@@H](CSCc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)O>C(C)(=O)O.C(C)(=O)OCC>O=C(Cc1ccccc1)N[C@@H](CS(=O)Cc1ccc(-c2ccc(-n3ccc4ccccc43)cc2)cc1)C(=O)O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-892c3d1426bd485caba0c509e21d7fd1
Brc1ccc(-c2cccc3c2oc2ccccc23)cc1.O=Cc1ccc(B(O)O)cc1>>O=Cc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
C([O-])([O-])=O.[Na+].[Na+].C(=O)C1=CC=C(C=C1)B(O)O.BrC1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1>>C1=CC=C(C=2OC3=C(C21)C=CC=C3)C3=CC=C(C=C3)C3=CC=C(C=C3)C=O
Br[c:7]1[cH:8][cH:9][c:10](-[c:11]2[cH:12][cH:13][cH:14][c:15]3[c:16]2[o:17][c:18]2[cH:19][cH:20][cH:21][cH:22][c:23]32)[cH:24][cH:25]1.OB(O)[c:6]1[cH:5][cH:4][c:3]([CH:2]=[O:1])[cH:27][cH:26]1>>[O:1]=[CH:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10](-[c:11]3[cH:12][cH:13][cH:14][c:15]4[c:16]3[o:17][c:18]3[cH:19]...
Brc1ccc(-c2cccc3c2oc2ccccc23)cc1.O=Cc1ccc(B(O)O)cc1
O=Cc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
null
null
C1(=CC=CC=C1)C.C(C)O
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:4]:[c:5]
null
[]
100
CELSIUS
null
null
A solution of 4-formylphenylboronic acid (0.9 g, 5.64 mmol) in ethanol (10 mL) was added to a stirred solution of the crude 4-(4-bromophenyl)-dibenzofuran (from the previous reaction) in toluene (40 mL). tetrakis-(Triphenylphosphine)palladium(0) (270 mg, 5 mol %) and 2N sodium carbonate (4.7 mL, 9.4 mmol) were added an...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1.c1ccc2c(c1)oc1ccccc12
HBr.B
C1(=CC=CC=C1)C.C(C)O
100
null
Brc1ccc(-c2cccc3c2oc2ccccc23)cc1.O=Cc1ccc(B(O)O)cc1>C1(=CC=CC=C1)C.C(C)O>O=Cc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-db804fd692aa4260a1641b4997e4a7cb
COC(=O)[C@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)OC(C)(C)C>>CC(C)(C)OC(=O)[C@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
[OH-].[Na+].COC([C@H](CSCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1)NC(=O)OC(C)(C)C)=O.CO.Cl>>C(C)(C)(C)OC(=O)[C@@H](C(=O)O)CSCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1
C[O:39][C:37]([C@@H:8](N[C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[CH2:9][S:10][CH2:11][c:12]1[cH:13][cH:14][c:15](-[c:16]2[cH:17][cH:18][c:19](-[c:20]3[cH:21][cH:22][cH:23][c:24]4[c:25]3[o:26][c:27]3[cH:28][cH:29][cH:30][cH:31][c:32]43)[cH:33][cH:34]2)[cH:35][cH:36]1)=[O:38]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5]...
COC(=O)[C@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)OC(C)(C)C
CC(C)(C)OC(=O)[C@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
null
null
O1CCCC1.O
Miscellaneous
OtherReaction
4db8e1a49fb6f0bcc9ee9f32b36a5f4a173f45727a0b6ffb6ccaf6e3e1f4602b
67ba51d9ece8d51253e171fb304ba5fff35ed9a0dd60b78a97bb1cfca9faa562
c1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[C@@H;D3;+0:4](-N-[C;H0;D3;+0:5](=[O;D1;H0:6])-[#8:7]-[C:8](-[C;D1;H3:9])(-[C;D1;H3:10])-[C;D1;H3:11])-[C:12]-[#16:13]>>[#16:13]-[C:12]-[C@H;D3;+0:4](-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1])-[C;H0;D3;+0:5](=[O;D1;H0:6])-[#8:7]-[C:8](-[C;D1;H3:9])(-[C;D1;H3:10])-[C;D1;H3:11]
null
[]
null
null
null
null
2N Sodium hydroxide solution (1.32 mL, 2.64 mmol) was added dropwise to a stirred solution of (2R)-methyl-2-tert-butoxycarbonylamino-3-(4′-dibenzofuran-4-yl-biphenyl-4-ylmethylsulfanyl)propionate (500 mg, 0.88 mmol) in tetrahydrofuran (15 mL) and methanol (3 mL). The clear reaction mixture was stirred at room temperatu...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ester
Carboxylic acid.Ester
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)oc1ccccc12
Other
O1CCCC1.O
null
null
COC(=O)[C@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)OC(C)(C)C>O1CCCC1.O>CC(C)(C)OC(=O)[C@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1c23e125befb4d0bb9066526dd17ea9b
CC(C)(C)OC(=O)[C@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O>>CC(C)(C)OC(=O)[C@H](CS(=O)Cc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
B1(OO1)[O-].O.O.O.O.[Na+].C(C)(C)(C)OC(=O)[C@@H](C(=O)O)CSCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1>>C(C)(C)(C)OC(=O)[C@@H](C(=O)O)CS(=O)CC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1
[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[C@H:8]([CH2:9][S:10][CH2:12][c:13]1[cH:14][cH:15][c:16](-[c:17]2[cH:18][cH:19][c:20](-[c:21]3[cH:22][cH:23][cH:24][c:25]4[c:26]3[o:27][c:28]3[cH:29][cH:30][cH:31][cH:32][c:33]43)[cH:34][cH:35]2)[cH:36][cH:37]1)[C:38](=[O:39])[OH:40]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C...
CC(C)(C)OC(=O)[C@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
CC(C)(C)OC(=O)[C@H](CS(=O)Cc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
null
null
C(C)(=O)O.C(C)(=O)OCC
Oxidation
Sulfanyl to sulfinyl
9edfaf6d72a81452ea8e3a1cdcb10a58409fff36608e97019e7273998b3d5373
f5f6bb6ca76a2267cd589767b4d67e7a17ab1ac383eeb6143dcd5d92e00e1b6a
c1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
[#8:1]-[C:2](=[O;D1;H0:3])-[C:4](-[C:5]-[S;H0;D2;+0:6]-[C:7]-[c:8])-[C:9](=[O;D1;H0:10])-[O;D1;H1:11]>>[#8:1]-[C:2](=[O;D1;H0:3])-[C:4](-[C:5]-[S;H0;D3;+0:6](=[O;D1;H0:12])-[C:7]-[c:8])-[C:9](=[O;D1;H0:10])-[O;D1;H1:11]
null
[]
40
CELSIUS
1
HOUR
Sodium perborate tetrahydrate (42 mg, 0.27 mmol) was added as a solid to a stirred solution of (2R)-2-tert-Butoxycarbonyl-3-(4′-dibenzofuran-4-yl-biphenyl-4-ylmethyl-sulfanyl)-propionic acid (150 mg, 0.27 mmol), in acetic acid (5 mL) at 40° C. This solution was stirred at 40° C. for 1 hour (HPLC control) and then dilut...
10.6084/m9.figshare.5104873.v1
null
Monosulfide
Sulfoxide
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)oc1ccccc12
null
C(C)(=O)O.C(C)(=O)OCC
40
1
CC(C)(C)OC(=O)[C@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O>C(C)(=O)O.C(C)(=O)OCC>CC(C)(C)OC(=O)[C@H](CS(=O)Cc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-fa161f9f8eea4eca8b8b0897739450c4
CC(C)(C)OC(=O)[C@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O>>CC(C)(C)OC(=O)[C@H](CS(=O)(=O)Cc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
B1(OO1)[O-].O.O.O.O.[Na+].C(C)(C)(C)OC(=O)[C@@H](C(=O)O)CSCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1>>C(C)(C)(C)OC(=O)[C@@H](C(=O)O)CS(=O)(=O)CC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1
[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[C@H:8]([CH2:9][S:10][CH2:13][c:14]1[cH:15][cH:16][c:17](-[c:18]2[cH:19][cH:20][c:21](-[c:22]3[cH:23][cH:24][cH:25][c:26]4[c:27]3[o:28][c:29]3[cH:30][cH:31][cH:32][cH:33][c:34]43)[cH:35][cH:36]2)[cH:37][cH:38]1)[C:39](=[O:40])[OH:41]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C...
CC(C)(C)OC(=O)[C@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
CC(C)(C)OC(=O)[C@H](CS(=O)(=O)Cc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
null
null
C(C)(=O)O.C(C)(=O)OCC
Oxidation
OtherReaction
20dd6d48007b4fe7cd760226f21413eb5e71e6468db112596c2e7ea4858c8ac1
5cedc1bf0f43f21d78a249521ecfcec19fc5ac4895c41eed0e84f0c2618149fa
c1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
[#8:1]-[C:2](=[O;D1;H0:3])-[C:4](-[C:5]-[S;H0;D2;+0:6]-[C:7]-[c:8])-[C:9](=[O;D1;H0:10])-[O;D1;H1:11]>>[#8:1]-[C:2](=[O;D1;H0:3])-[C:4](-[C:5]-[S;H0;D4;+0:6](=[O;D1;H0:12])(=[O;D1;H0:13])-[C:7]-[c:8])-[C:9](=[O;D1;H0:10])-[O;D1;H1:11]
89.6
[{"value": 87.0, "product": "C(C)(C)(C)OC(=O)[C@@H](C(=O)O)CS(=O)(=O)CC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 89.6, "product": "C(C)(C)(C)OC(=O)[C@@H](C(=O)O)CS(=O)(=O)CC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1", "details": "CALCULATEDPE...
40
CELSIUS
2
HOUR
Sodium perborate tetrahydrate (105 mg, 0.68 mmol) was added as a solid to a stirred solution of (2R)-2-tert-Butoxycarbonyl-3-(4′-dibenzofuran-4-yl-biphenyl-4-ylmethyl-sulfanyl)-propionic acid (150 mg, 0.27 mmol), in acetic acid (10 mL) at 50° C. This solution was stirred at 40° C. for 2 hours (HPLC control) and then di...
10.6084/m9.figshare.5104873.v1
null
Monosulfide
Sulfone
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)oc1ccccc12
null
C(C)(=O)O.C(C)(=O)OCC
40
2
CC(C)(C)OC(=O)[C@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O>C(C)(=O)O.C(C)(=O)OCC>CC(C)(C)OC(=O)[C@H](CS(=O)(=O)Cc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a380b04f2a6540cb8354a547ad1b0d5c
COC(=O)[C@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)OC(C)(C)C>>COC(=O)[C@@H](N)CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
[Si](C)(C)(C)I.COC([C@H](CSCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1)NC(=O)OC(C)(C)C)=O.C([O-])(O)=O.[Na+]>>COC([C@H](CSCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1)N)=O
CC(C)(C)OC(=O)[NH:6][C@H:5]([C:3]([O:2][CH3:1])=[O:4])[CH2:7][S:8][CH2:9][c:10]1[cH:11][cH:12][c:13](-[c:14]2[cH:15][cH:16][c:17](-[c:18]3[cH:19][cH:20][cH:21][c:22]4[c:23]3[o:24][c:25]3[cH:26][cH:27][cH:28][cH:29][c:30]43)[cH:31][cH:32]2)[cH:33][cH:34]1>>[CH3:1][O:2][C:3](=[O:4])[C@@H:5]([NH2:6])[CH2:7][S:8][CH2:9][c:...
COC(=O)[C@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)OC(C)(C)C
COC(=O)[C@@H](N)CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
null
null
O.C(Cl)Cl
Reduction
Hydrogenolysis of amides/imides/carbamates
3c33dd2a2d355ee5ba0287367e209aa147a39aa00607f0c95fb2bf1ade45d014
c5b5dffe7dd8beebdc1baa8b5b05300a9f7079e65dcfd42ade6f8a77ff09537d
c1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[C:2](-[C:3])-[C:4](=[O;D1;H0:5])-[#8:6]-[C;D1;H3:7]>>[C:3]-[C:2](-[NH2;D1;+0:1])-[C:4](=[O;D1;H0:5])-[#8:6]-[C;D1;H3:7]
null
[]
null
null
25
MINUTE
TMS-I (870 mg, 0.63 mL, 4.35 mmol) was added dropwise to a stirred solution of (2R)-methyl-2-tert-butoxycarbonylamino-3-(4′-dibenzofuran-4-yl-biphenyl-4-ylmethyl-sulfanyl)-propionate (2.24 g, 3.96 mmol) in anhydrous methylene chloride (50 mL). The reaction mixture was stirred at room temperature for 20-30 mins (TLC con...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Primary amine
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)oc1ccccc12
HO-
O.C(Cl)Cl
null
0.416667
COC(=O)[C@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)OC(C)(C)C>O.C(Cl)Cl>COC(=O)[C@@H](N)CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-990557efc3754733aed4ec56f27a6846
COC(=O)[C@@H](N)CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1>>N[C@@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
[OH-].[Na+].COC([C@H](CSCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1)N)=O.Cl>>N[C@H](C(=O)O)CSCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1
C[O:33][C:31]([C@@H:2]([NH2:1])[CH2:3][S:4][CH2:5][c:6]1[cH:7][cH:8][c:9](-[c:10]2[cH:11][cH:12][c:13](-[c:14]3[cH:15][cH:16][cH:17][c:18]4[c:19]3[o:20][c:21]3[cH:22][cH:23][cH:24][cH:25][c:26]43)[cH:27][cH:28]2)[cH:29][cH:30]1)=[O:32]>>[NH2:1][C@@H:2]([CH2:3][S:4][CH2:5][c:6]1[cH:7][cH:8][c:9](-[c:10]2[cH:11][cH:12][c...
COC(=O)[C@@H](N)CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
N[C@@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
null
null
O1CCCC1.CO
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
86
[{"value": 86.0, "product": "N[C@H](C(=O)O)CSCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 85.6, "product": "N[C@H](C(=O)O)CSCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
2N Sodium hydroxide (0.5 mL) was added to a stirred solution of the amino methyl ester, (2R)-Methyl-2-Amino-3-(4′-dibenzofuran-4-ylbipheny-4-ylmethylsulfanyl)-propionate (100 mg) in a mixture of tetrahydrofuran (5 mL) and methanol (1 mL). The solution was stirred for 1 hour and then acidified to pH 3 with 2N hydrochlor...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)oc1ccccc12
Other
O1CCCC1.CO
null
1
COC(=O)[C@@H](N)CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1>O1CCCC1.CO>N[C@@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-276b12e917a04c8181274b48fa1e325e
CC(C)(C)OC(=O)N=C(NC(=O)OC(C)(C)C)N[C@@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O>>N=C(N)N[C@@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
FC(C(=O)O)(F)F.C(C)(C)(C)OC(=O)N=C(N[C@H](C(=O)O)CSCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1)NC(=O)OC(C)(C)C>>C1=CC=C(C=2OC3=C(C21)C=CC=C3)C3=CC=C(C=C3)C3=CC=C(C=C3)CSC[C@@H](C(=O)O)NC(=N)N
CC(C)(C)OC(=O)[N:1]=[C:2]([NH:3]C(=O)OC(C)(C)C)[NH:4][C@@H:5]([CH2:6][S:7][CH2:8][c:9]1[cH:10][cH:11][c:12](-[c:13]2[cH:14][cH:15][c:16](-[c:17]3[cH:18][cH:19][cH:20][c:21]4[c:22]3[o:23][c:24]3[cH:25][cH:26][cH:27][cH:28][c:29]43)[cH:30][cH:31]2)[cH:32][cH:33]1)[C:34](=[O:35])[OH:36]>>[NH:1]=[C:2]([NH2:3])[NH:4][C@@H:5...
CC(C)(C)OC(=O)N=C(NC(=O)OC(C)(C)C)N[C@@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
N=C(N)N[C@@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
null
null
ClCCl
Reduction
Boc amine deprotection of guanidine
9766f6229fee762ffca87ed66a89907c51d08c86b25c0988ddb4d7c2e968882c
8451d9ce44c8e1c8be0145c0e21ac06b9d8969460bd0e7e8568f82462587cbce
c1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
C-C(-C)(-C)-O-C(=O)-[N;H0;D2;+0:1]=[C:2](-[#7:3])-[NH;D2;+0:4]-C(=O)-O-C(-C)(-C)-C>>[#7:3]-[C:2](-[NH2;D1;+0:4])=[NH;D1;+0:1]
99
[{"value": 99.0, "product": "C1=CC=C(C=2OC3=C(C21)C=CC=C3)C3=CC=C(C=C3)C3=CC=C(C=C3)CSC[C@@H](C(=O)O)NC(=N)N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 98.1, "product": "C1=CC=C(C=2OC3=C(C21)C=CC=C3)C3=CC=C(C=C3)C3=CC=C(C=C3)CSC[C@@H](C(=O)O)NC(=N)N", "details": "CALCULATEDPERCENTYIELD", "is_desired":...
null
null
4
HOUR
Trifluoroacetic acid (2 mL) was added to a stirred solution of (2R)-2-[2,3-bis-(tert-butoxycarbonyl)guanidino]-3-(4′-dibenzofuran-4-yl-biphenyl-4-ylmethylsulfanyl)-propionic acid (250 mg, 0.36 mmol) in anhydrous dichloromethane (10 mL). The reaction was stirred for 4 hours (HPLC control) and then concentrated in vacuo....
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Ether.Boc.Boc
Primary amine
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)oc1ccccc12
HO-
ClCCl
null
4
CC(C)(C)OC(=O)N=C(NC(=O)OC(C)(C)C)N[C@@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O>ClCCl>N=C(N)N[C@@H](CSCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4146c15b24c54bf889fefafdbcae8ab2
O=Cc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1>>OCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1
C(C1=CC=CC=C1)C=1OC2=C(C1C1=CC=C(C=C1)C1=CC=C(C=C1)C=O)C=CC=C2.[BH4-].[Na+].O>>C(C1=CC=CC=C1)C=1OC2=C(C1C1=CC=C(C=C1)C1=CC=C(C=C1)CO)C=CC=C2
[O:1]=[CH:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10](-[c:11]3[c:12]([CH2:13][c:14]4[cH:15][cH:16][cH:17][cH:18][cH:19]4)[o:20][c:21]4[cH:22][cH:23][cH:24][cH:25][c:26]34)[cH:27][cH:28]2)[cH:29][cH:30]1>>[OH:1][CH2:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10](-[c:11]3[c:12]([CH2:13][c:14]4[cH:15][cH:16][...
O=Cc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1
OCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1
null
null
O1CCCC1.C(C)O
Reduction
Reduction of aldehydes and ketones to alcohols
e7895795cd3f75445716c94697823c5929dcd4b5344525875fe75d36bca2f9d7
21bb81d5469aaaca71ab12c186bea4016451717fad8780cf288858a7d8fbc55a
c1ccc(Cc2oc3ccccc3c2-c2ccc(-c3ccccc3)cc2)cc1
[O;H0;D1;+0:1]=[CH;D2;+0:2]-[c:3](:[c:4]):[c:5]>>[OH;D1;+0:1]-[CH2;D2;+0:2]-[c:3](:[c:4]):[c:5]
99.7
[{"value": 99.0, "product": "C(C1=CC=CC=C1)C=1OC2=C(C1C1=CC=C(C=C1)C1=CC=C(C=C1)CO)C=CC=C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 99.7, "product": "C(C1=CC=CC=C1)C=1OC2=C(C1C1=CC=C(C=C1)C1=CC=C(C=C1)CO)C=CC=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a solution of 4′-(2-benzylbenzofuran-3-yl)biphenyl-4-carbaldehyde (5.0 g, 12.9 mmol) in ethanol (100 mL) and tetrahydrofuran (25 mL) was added sodium borohydride (980 mg, 25.8 mmol) as a solid in 3 portions. The reaction was stirred at room temperature for 1 hour (TLC control) and then poured into water (100 mL) and...
10.6084/m9.figshare.5104873.v1
null
Aldehyde
Primary alcohol
null
null
c1ccccc1.c1ccccc1.c1ccccc1.c1ccc2occc2c1
null
O1CCCC1.C(C)O
null
1
O=Cc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1>O1CCCC1.C(C)O>OCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-cf2c72086a0e4d198532d5ad07313887
BrP(Br)(c1ccccc1)(c1ccccc1)c1ccccc1.OCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1>>BrCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1
O.C(C1=CC=CC=C1)C=1OC2=C(C1C1=CC=C(C=C1)C1=CC=C(C=C1)CO)C=CC=C2.BrP(C1=CC=CC=C1)(C1=CC=CC=C1)(C1=CC=CC=C1)Br>>C(C1=CC=CC=C1)C=1OC2=C(C1C1=CC=C(C=C1)C1=CC=C(C=C1)CBr)C=CC=C2
BrP(c1ccccc1)(c1ccccc1)(c1ccccc1)[Br:1].O[CH2:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10](-[c:11]3[c:12]([CH2:13][c:14]4[cH:15][cH:16][cH:17][cH:18][cH:19]4)[o:20][c:21]4[cH:22][cH:23][cH:24][cH:25][c:26]34)[cH:27][cH:28]2)[cH:29][cH:30]1>>[Br:1][CH2:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10](-[c:11]3[...
BrP(Br)(c1ccccc1)(c1ccccc1)c1ccccc1.OCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1
BrCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1
null
null
C(C)#N
Functional Group Interconversion
OtherReaction
8872f2fae3cc46ec19a3bd8f9f9484c21a537e6d42617740a795333c61c3afc4
cbf41c7cf9fe6b47a243b1674d74ed5bf46a151f7f3a71d206e23176e158facf
c1ccc(Cc2oc3ccccc3c2-c2ccc(-c3ccccc3)cc2)cc1
Br-P(-[Br;H0;D1;+0:1])(-c1:c:c:c:c:c:1)(-c1:c:c:c:c:c:1)-c1:c:c:c:c:c:1.O-[CH2;D2;+0:2]-[c:3](:[c:4]):[c:5]>>[Br;H0;D1;+0:1]-[CH2;D2;+0:2]-[c:3](:[c:4]):[c:5]
87
[{"value": 87.0, "product": "C(C1=CC=CC=C1)C=1OC2=C(C1C1=CC=C(C=C1)C1=CC=C(C=C1)CBr)C=CC=C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 86.5, "product": "C(C1=CC=CC=C1)C=1OC2=C(C1C1=CC=C(C=C1)C1=CC=C(C=C1)CBr)C=CC=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
To a solution of 4′-(2-benzylbenzofuran-3-yl)biphenyl-4-methanol (5.01 g, 12.7 mmol) in anhydrous acetonitrile (75 mL) was added dibromotriphenylphosphorane (5.45 g, 12.7 mmol) as a solid portionwise over 15 mins. The reaction was stirred for 2 hours (TLC control) and then poured into water (100 mL) and extracted with ...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Primary halide
c1ccccc1.c1ccccc1.c1ccccc1
null
c1ccccc1.c1ccccc1.c1ccccc1.c1ccc2occc2c1
HBr
C(C)#N
null
2
BrP(Br)(c1ccccc1)(c1ccccc1)c1ccccc1.OCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1>C(C)#N>BrCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a0d70d242b6649fd8d306f20012c629b
BrCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1.COC(=O)[C@H](CS)NC(=O)OC(C)(C)C>>COC(=O)[C@H](CSCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1)NC(=O)OC(C)(C)C
O.COC([C@@H](NC(=O)OC(C)(C)C)CS)=O.C(C1=CC=CC=C1)C=1OC2=C(C1C1=CC=C(C=C1)C1=CC=C(C=C1)CBr)C=CC=C2.C([O-])([O-])=O.[Cs+].[Cs+]>>COC([C@H](CSCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=C(OC2=C1C=CC=C2)CC2=CC=CC=C2)NC(=O)OC(C)(C)C)=O
Br[CH2:8][c:9]1[cH:10][cH:11][c:12](-[c:13]2[cH:14][cH:15][c:16](-[c:17]3[c:18]([CH2:19][c:20]4[cH:21][cH:22][cH:23][cH:24][cH:25]4)[o:26][c:27]4[cH:28][cH:29][cH:30][cH:31][c:32]34)[cH:33][cH:34]2)[cH:35][cH:36]1.[CH3:1][O:2][C:3](=[O:4])[C@H:5]([CH2:6][SH:7])[NH:37][C:38](=[O:39])[O:40][C:41]([CH3:42])([CH3:43])[CH3:...
BrCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1.COC(=O)[C@H](CS)NC(=O)OC(C)(C)C
COC(=O)[C@H](CSCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1)NC(=O)OC(C)(C)C
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
thioether_nucl_sub
77cd742b5ba20df0e225494f6e5f3d958ee82ce9a1b16fd99a2d9f8350b4fdc8
b05f7dda7dad719ae1868a84c33eeaf5bf649036fc64173cf4774a5eb4d70181
c1ccc(Cc2oc3ccccc3c2-c2ccc(-c3ccccc3)cc2)cc1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[#8:5]-[C:6](=[O;D1;H0:7])-[C:8]-[C:9]-[SH;D1;+0:10]>>[#8:5]-[C:6](=[O;D1;H0:7])-[C:8]-[C:9]-[S;H0;D2;+0:10]-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
92.7
[{"value": 92.0, "product": "COC([C@H](CSCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=C(OC2=C1C=CC=C2)CC2=CC=CC=C2)NC(=O)OC(C)(C)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 92.7, "product": "COC([C@H](CSCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=C(OC2=C1C=CC=C2)CC2=CC=CC=C2)NC(=O)OC(C)(C)C)=O", "details": "CALCULATEDPERCENTY...
null
null
2
HOUR
N-Boc-L-Cysteine methyl ester (260 mg, 0.23 mL, 1.1 mmol) was added dropwise to a stirred suspension of 2-Benzyl-3-(4′-bromomethylbiphen-4-yl)benzofuran (500 mg, 1.1 mmol) and cesium carbonate (720 mg, 2.21 mmol) in anhydrous dimethylformamide (20 mL). The reaction was stirred at room temperature for 2 hrs (TLC control...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aliphatic thiol
Monosulfide
null
null
c1ccccc1.c1ccccc1.c1ccccc1.c1ccc2occc2c1
HBr
CN(C=O)C
null
2
BrCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1.COC(=O)[C@H](CS)NC(=O)OC(C)(C)C>CN(C=O)C>COC(=O)[C@H](CSCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1)NC(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7d8b9ee1091948778ebfa982fa423205
COC(=O)[C@H](CSCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1)NC(=O)OC(C)(C)C>>CC(C)(C)O[C@](CSCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1)(N=C=O)C(=O)O
[OH-].[Na+].COC([C@H](CSCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=C(OC2=C1C=CC=C2)CC2=CC=CC=C2)NC(=O)OC(C)(C)C)=O.Cl>>C(C1=CC=CC=C1)C=1OC2=C(C1C1=CC=C(C3=CC=C(C=C3)CSC[C@@](C(=O)O)(OC(C)(C)C)N=C=O)C=C1)C=CC=C2
C[O:43][C:41]([C@H:6]([CH2:7][S:8][CH2:9][c:10]1[cH:11][cH:12][c:13](-[c:14]2[cH:15][cH:16][c:17](-[c:18]3[c:19]([CH2:20][c:21]4[cH:22][cH:23][cH:24][cH:25][cH:26]4)[o:27][c:28]4[cH:29][cH:30][cH:31][cH:32][c:33]34)[cH:34][cH:35]2)[cH:36][cH:37]1)[NH:38][C:39]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:40])=[O:42]>>[CH3:1...
COC(=O)[C@H](CSCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1)NC(=O)OC(C)(C)C
CC(C)(C)O[C@](CSCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1)(N=C=O)C(=O)O
null
null
O1CCCC1.CO
Miscellaneous
OtherReaction
bddd03b924038931273bed81e8862363f2f3e48dd28556c3a68c5d8c7a1d08f8
cc5b0328a1c3fc37b615ae32d720dd8bdc1cf4d0986d2062548d49debb17cf49
c1ccc(Cc2oc3ccccc3c2-c2ccc(-c3ccccc3)cc2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[C@H;D3;+0:4](-[C:5]-[#16:6])-[NH;D2;+0:7]-[C;H0;D3;+0:8](=[O;D1;H0:9])-[O;H0;D2;+0:10]-[C:11](-[C;D1;H3:12])(-[C;D1;H3:13])-[C;D1;H3:14]>>[#16:6]-[C:5]-[C@;H0;D4;+0:4](-[N;H0;D2;+0:7]=[C;H0;D2;+0:8]=[O;D1;H0:9])(-[O;H0;D2;+0:10]-[C:11](-[C;D1;H3:12])(-[C;D1;H3:13])-[C;D1;H3:14])-[C...
84
[{"value": 84.0, "product": "C(C1=CC=CC=C1)C=1OC2=C(C1C1=CC=C(C3=CC=C(C=C3)CSC[C@@](C(=O)O)(OC(C)(C)C)N=C=O)C=C1)C=CC=C2", "details": "PERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
1N Sodium hydroxide (2 mL) was added to a stirred solution of (2R)-methyl-3-[4′-(2-benzylbenzofuran-3-yl)biphen-4-ylmethylsulfanyl]-2-tert-butoxycarbonylamino-propionate (100 mg) in a mixture of tetrahydrofuran (6 mL) and methanol (2 mL). The solution was stirred for 1 hour and then acidified to pH 3 with 1N hydrochlor...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ester
Carboxylic acid.Ether.Isocyanate
null
null
c1ccccc1.c1ccccc1.c1ccccc1.c1ccc2occc2c1
Other
O1CCCC1.CO
null
1
COC(=O)[C@H](CSCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1)NC(=O)OC(C)(C)C>O1CCCC1.CO>CC(C)(C)O[C@](CSCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1)(N=C=O)C(=O)O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-baf9dffcf2204eb8856112afb74bef5b
CC(C)(C)OC(=O)N[C@@H](CSCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1)C(=O)O>>CC(C)(C)OC(=O)N[C@@H](CS(=O)(=O)Cc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1)C(=O)O
B1(OO1)[O-].O.O.O.O.[Na+].C(C1=CC=CC=C1)C=1OC2=C(C1C1=CC=C(C3=CC=C(C=C3)CSC[C@@H](C(=O)O)NC(=O)OC(C)(C)C)C=C1)C=CC=C2>>C(C1=CC=CC=C1)C=1OC2=C(C1C1=CC=C(C3=CC=C(C=C3)CS(=O)(=O)C[C@@H](C(=O)O)NC(=O)OC(C)(C)C)C=C1)C=CC=C2
[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[NH:8][C@@H:9]([CH2:10][S:11][CH2:14][c:15]1[cH:16][cH:17][c:18](-[c:19]2[cH:20][cH:21][c:22](-[c:23]3[c:24]([CH2:25][c:26]4[cH:27][cH:28][cH:29][cH:30][cH:31]4)[o:32][c:33]4[cH:34][cH:35][cH:36][cH:37][c:38]34)[cH:39][cH:40]2)[cH:41][cH:42]1)[C:43](=[O:44])[OH:45]>>[CH3:...
CC(C)(C)OC(=O)N[C@@H](CSCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1)C(=O)O
CC(C)(C)OC(=O)N[C@@H](CS(=O)(=O)Cc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1)C(=O)O
null
null
C(C)(=O)O.C(C)(=O)OCC
Oxidation
OtherReaction
20dd6d48007b4fe7cd760226f21413eb5e71e6468db112596c2e7ea4858c8ac1
5cedc1bf0f43f21d78a249521ecfcec19fc5ac4895c41eed0e84f0c2618149fa
c1ccc(Cc2oc3ccccc3c2-c2ccc(-c3ccccc3)cc2)cc1
[O;D1;H0:1]=[C:2](-[O;D1;H1:3])-[C:4]-[C:5]-[S;H0;D2;+0:6]-[C:7]-[c:8]>>[O;D1;H0:9]=[S;H0;D4;+0:6](=[O;D1;H0:10])(-[C:5]-[C:4]-[C:2](=[O;D1;H0:1])-[O;D1;H1:3])-[C:7]-[c:8]
92
[{"value": 92.0, "product": "C(C1=CC=CC=C1)C=1OC2=C(C1C1=CC=C(C3=CC=C(C=C3)CS(=O)(=O)C[C@@H](C(=O)O)NC(=O)OC(C)(C)C)C=C1)C=CC=C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 92.0, "product": "C(C1=CC=CC=C1)C=1OC2=C(C1C1=CC=C(C3=CC=C(C=C3)CS(=O)(=O)C[C@@H](C(=O)O)NC(=O)OC(C)(C)C)C=C1)C=CC=C2", "details":...
40
CELSIUS
2
HOUR
Sodium perborate tetrahydrate (320 mg, 2.1 mmol) was added as a solid to a stirred solution of (2R)-3-[4′-(2-benzylbenzofuran-3-yl)biphen-4-ylmethylsulfanyl]-2-tert-butoxycarbonylamino-propionic acid (440 mg, 0.74 mmol) in acetic acid (10 mL) at 40° C. This solution was stirred at 40° C. for 2 hours (HPLC control) and ...
10.6084/m9.figshare.5104873.v1
null
Monosulfide
Sulfone
null
null
c1ccccc1.c1ccccc1.c1ccccc1.c1ccc2occc2c1
null
C(C)(=O)O.C(C)(=O)OCC
40
2
CC(C)(C)OC(=O)N[C@@H](CSCc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1)C(=O)O>C(C)(=O)O.C(C)(=O)OCC>CC(C)(C)OC(=O)N[C@@H](CS(=O)(=O)Cc1ccc(-c2ccc(-c3c(Cc4ccccc4)oc4ccccc34)cc2)cc1)C(=O)O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f9e0f04e7b404f6dbea27116ba7ebe2e
CS(=O)(=O)Cl.OCc1ccc(-c2nc(-c3ccccc3)cc(-c3ccccc3)n2)cc1>>CS(=O)(=O)OCc1ccc(-c2nc(-c3ccccc3)cc(-c3ccccc3)n2)cc1
C1(=CC=CC=C1)C1=NC(=NC(=C1)C1=CC=CC=C1)C1=CC=C(C=C1)CO.C(C)N(CC)CC.CS(=O)(=O)Cl>>C1(=CC=CC=C1)C1=NC(=NC(=C1)C1=CC=CC=C1)C1=CC=C(COS(=O)(=O)C)C=C1
Cl[S:2]([CH3:1])(=[O:3])=[O:4].[OH:5][CH2:6][c:7]1[cH:8][cH:9][c:10](-[c:11]2[n:12][c:13](-[c:14]3[cH:15][cH:16][cH:17][cH:18][cH:19]3)[cH:20][c:21](-[c:22]3[cH:23][cH:24][cH:25][cH:26][cH:27]3)[n:28]2)[cH:29][cH:30]1>>[CH3:1][S:2](=[O:3])(=[O:4])[O:5][CH2:6][c:7]1[cH:8][cH:9][c:10](-[c:11]2[n:12][c:13](-[c:14]3[cH:15]...
CS(=O)(=O)Cl.OCc1ccc(-c2nc(-c3ccccc3)cc(-c3ccccc3)n2)cc1
CS(=O)(=O)OCc1ccc(-c2nc(-c3ccccc3)cc(-c3ccccc3)n2)cc1
null
null
C(Cl)Cl
Acylation
Formation of Sulfonic Esters
2fa969eb2c954bb96793348a1b2335ec63fbd290dadec6e3e02295e1768e64cf
cb77b899e4adf980b1def97230ef2861660fd7f9602260ec64747d9afd3a795a
c1ccc(-c2cc(-c3ccccc3)nc(-c3ccccc3)n2)cc1
Cl-[S;H0;D4;+0:1](-[C;D1;H3:2])(=[O;D1;H0:3])=[O;D1;H0:4].[OH;D1;+0:5]-[C:6]-[c:7]>>[C;D1;H3:2]-[S;H0;D4;+0:1](=[O;D1;H0:3])(=[O;D1;H0:4])-[O;H0;D2;+0:5]-[C:6]-[c:7]
null
[]
0
CELSIUS
2
HOUR
A solution of [4-(4,6-diphenylpyrimidin-2-yl)-phenyl]methanol, 0.38 g (1.11 mmol), triethylamine, 0.34 mL (2.45 mmol), and 6 mL of methylene chloride was cooled to 0° C. via ice-water bath. Methanesulfonyl chloride, 0.10 mL (1.23 mmol) was added dropwise over minutes. The solution stirred for 2 h at 0° C. The solution ...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Sulfonyl halide
Mesylate
null
null
c1ccccc1.c1cncnc1.c1ccccc1.c1ccccc1
HCl
C(Cl)Cl
0
2
CS(=O)(=O)Cl.OCc1ccc(-c2nc(-c3ccccc3)cc(-c3ccccc3)n2)cc1>C(Cl)Cl>CS(=O)(=O)OCc1ccc(-c2nc(-c3ccccc3)cc(-c3ccccc3)n2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0d421daf3a5f455eb4058ba1413d1e40
COC(=O)[C@H](CS)NC(=O)OC(C)(C)C.CS(=O)(=O)OCc1ccc(-c2nc(-c3ccccc3)cc(-c3ccccc3)n2)cc1>>COC(=O)C(CSCc1ccc(-c2nc(-c3ccccc3)cc(-c3ccccc3)n2)cc1)NC(=O)OC(C)(C)C
C1(=CC=CC=C1)C1=NC(=NC(=C1)C1=CC=CC=C1)C1=CC=C(COS(=O)(=O)C)C=C1.COC([C@@H](NC(=O)OC(C)(C)C)CS)=O.C([O-])([O-])=O.[Cs+].[Cs+].CN(C=O)C>>COC(C(CSCC1=CC=C(C=C1)C1=NC(=CC(=N1)C1=CC=CC=C1)C1=CC=CC=C1)NC(=O)OC(C)(C)C)=O
[CH3:1][O:2][C:3](=[O:4])[C@H:5]([CH2:6][SH:7])[NH:33][C:34](=[O:35])[O:36][C:37]([CH3:38])([CH3:39])[CH3:40].CS(=O)(=O)O[CH2:8][c:9]1[cH:10][cH:11][c:12](-[c:13]2[n:14][c:15](-[c:16]3[cH:17][cH:18][cH:19][cH:20][cH:21]3)[cH:22][c:23](-[c:24]3[cH:25][cH:26][cH:27][cH:28][cH:29]3)[n:30]2)[cH:31][cH:32]1>>[CH3:1][O:2][C:...
COC(=O)[C@H](CS)NC(=O)OC(C)(C)C.CS(=O)(=O)OCc1ccc(-c2nc(-c3ccccc3)cc(-c3ccccc3)n2)cc1
COC(=O)C(CSCc1ccc(-c2nc(-c3ccccc3)cc(-c3ccccc3)n2)cc1)NC(=O)OC(C)(C)C
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
5ef6153311053d1fb9aeb0863ac740df1693ec5dc2fd63b54be9bba291d50d91
5d51471fb107f265fe2b725316ea74298d6b5b18b8910d02b969c8ad6fbd6b39
c1ccc(-c2cc(-c3ccccc3)nc(-c3ccccc3)n2)cc1
C-S(=O)(=O)-O-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[#8:5]-[C:6](=[O;D1;H0:7])-[C:8]-[C:9]-[SH;D1;+0:10]>>[#8:5]-[C:6](=[O;D1;H0:7])-[C:8]-[C:9]-[S;H0;D2;+0:10]-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
4
HOUR
A mixture of Methanesulfonic acid 4-(4,6-diphenylpyrimidin-2-yl)-benzyl ester, 0.15 g (0.36 mmol), N-(tert-Butoxycarbonyl)-L-cysteine methyl ester, 0.08 mL (0.36 mmol), cesium carbonate, 235 mg (0.72 mmol), and 10 mL of N,N-dimethylformamide was stirred at room temperature for 4 h. The mixture was diluted with 10 mL of...
10.6084/m9.figshare.5104873.v1
null
Mesylate.Aliphatic thiol
Monosulfide
null
null
c1ccccc1.c1cncnc1.c1ccccc1.c1ccccc1
MsOH.HO-
O
null
4
COC(=O)[C@H](CS)NC(=O)OC(C)(C)C.CS(=O)(=O)OCc1ccc(-c2nc(-c3ccccc3)cc(-c3ccccc3)n2)cc1>O>COC(=O)C(CSCc1ccc(-c2nc(-c3ccccc3)cc(-c3ccccc3)n2)cc1)NC(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d07a2c718bb74917ab2d64f61b49b0ea
COC(=O)C(CSCc1ccc(-c2nc(-c3ccccc3)cc(-c3ccccc3)n2)cc1)NC(=O)OC(C)(C)C>>CC(C)(C)OC(=O)NC(CSCc1ccc(-c2nc(-c3ccccc3)cc(-c3ccccc3)n2)cc1)C(=O)O
COC(C(CSCC1=CC=C(C=C1)C1=NC(=CC(=N1)C1=CC=CC=C1)C1=CC=CC=C1)NC(=O)OC(C)(C)C)=O.CO.[OH-].[K+]>>C(C)(C)(C)OC(=O)NC(C(=O)O)CSCC1=CC=C(C=C1)C1=NC(=CC(=N1)C1=CC=CC=C1)C1=CC=CC=C1
C[O:39][C:37]([CH:9]([NH:8][C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[CH2:10][S:11][CH2:12][c:13]1[cH:14][cH:15][c:16](-[c:17]2[n:18][c:19](-[c:20]3[cH:21][cH:22][cH:23][cH:24][cH:25]3)[cH:26][c:27](-[c:28]3[cH:29][cH:30][cH:31][cH:32][cH:33]3)[n:34]2)[cH:35][cH:36]1)=[O:38]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][...
COC(=O)C(CSCc1ccc(-c2nc(-c3ccccc3)cc(-c3ccccc3)n2)cc1)NC(=O)OC(C)(C)C
CC(C)(C)OC(=O)NC(CSCc1ccc(-c2nc(-c3ccccc3)cc(-c3ccccc3)n2)cc1)C(=O)O
null
null
O1CCCC1.O
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(-c2cc(-c3ccccc3)nc(-c3ccccc3)n2)cc1
C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
null
[]
null
null
1
HOUR
To a solution of 2-tert-Butoxy carbonylamino-3-[4-(4,6-diphenylpyrimidin-2-yl)-benzylsulfanyl]-propionic acid methyl ester, 0.18 g (0.32 mmol) in 10 mL of tetrahydrofuran and 5 mL of methanol was added 1.62 mL of 1.0M aq. KOH. The solution was stirred for 1 h at room temperature. The solution was diluted with 10 mL of ...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1cncnc1.c1ccccc1.c1ccccc1
Other
O1CCCC1.O
null
1
COC(=O)C(CSCc1ccc(-c2nc(-c3ccccc3)cc(-c3ccccc3)n2)cc1)NC(=O)OC(C)(C)C>O1CCCC1.O>CC(C)(C)OC(=O)NC(CSCc1ccc(-c2nc(-c3ccccc3)cc(-c3ccccc3)n2)cc1)C(=O)O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f8b428ec23fd4237a150471823319346
COC(=O)c1ccc(I)cc1.OB(O)c1ccc(Br)cc1>>COC(=O)c1ccc(-c2ccc(Br)cc2)cc1
C(=O)([O-])[O-].[Na+].[Na+].C(C)O.IC1=CC=C(C(=O)OC)C=C1.BrC1=CC=C(C=C1)B(O)O>>COC(=O)C1=CC=C(C=C1)C1=CC=C(C=C1)Br
I[c:8]1[cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:17][cH:16]1.OB(O)[c:9]1[cH:10][cH:11][c:12]([Br:13])[cH:14][cH:15]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8](-[c:9]2[cH:10][cH:11][c:12]([Br:13])[cH:14][cH:15]2)[cH:16][cH:17]1
COC(=O)c1ccc(I)cc1.OB(O)c1ccc(Br)cc1
COC(=O)c1ccc(-c2ccc(Br)cc2)cc1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
C1(=CC=CC=C1)C.C(C)(=O)OCC
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccccc2)cc1
I-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:8]:[c:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9]:[c:10]
null
[]
80
CELSIUS
null
null
A mixture of methyl 4-iodobenzoate, 9.38 g (35.8 mmol), 4-bromophenylboronic acid 7.18 g (35.8 mmol), Pd(PPh3)4, 2.07 g (1.79 mmol), in 180 mL of toluene and 100 mL of ethanol was heated to obtain a clear solution. To the solution was added 30 mL of 4.0M aq. Na2CO3. The reaction mixture refluxed for 4 h at 80° C. The m...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
HI.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C1(=CC=CC=C1)C.C(C)(=O)OCC
80
null
COC(=O)c1ccc(I)cc1.OB(O)c1ccc(Br)cc1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C1(=CC=CC=C1)C.C(C)(=O)OCC>COC(=O)c1ccc(-c2ccc(Br)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0d8b78dd1e8e4d319a4cdeb5fdbd1fab
COC(=O)c1ccc(-c2ccc(Br)cc2)cc1>>OCc1ccc(-c2ccc(Br)cc2)cc1
COC(=O)C1=CC=C(C=C1)C1=CC=C(C=C1)Br.[H-].[Al+3].[Li+].[H-].[H-].[H-]>>BrC1=CC=C(C=C1)C1=CC=C(C=C1)CO
CO[C:2](=[O:1])[c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([Br:11])[cH:12][cH:13]2)[cH:14][cH:15]1>>[OH:1][CH2:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([Br:11])[cH:12][cH:13]2)[cH:14][cH:15]1
COC(=O)c1ccc(-c2ccc(Br)cc2)cc1
OCc1ccc(-c2ccc(Br)cc2)cc1
null
null
O1CCCC1
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
c1ccc(-c2ccccc2)cc1
C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3](:[c:4]):[c:5]>>[OH;D1;+0:2]-[CH2;D2;+0:1]-[c:3](:[c:4]):[c:5]
null
[]
0
CELSIUS
1
HOUR
A solution of 4′-Bromo-biphenyl-4-carboxylic acid methyl ester, 7.8 g (27.9 mmol) in 150 mL of tetrahydrofuran was cooled to 0° C. via ice-water bath. Lithium aluminum hydride, 1.1 g (27.9 mmol) was added to the solution in one portion. The reaction mixture stirred at 0° C. for 1 h. The mixture was slowly quenched with...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
c1ccccc1.c1ccccc1
Other
O1CCCC1
0
1
COC(=O)c1ccc(-c2ccc(Br)cc2)cc1>O1CCCC1>OCc1ccc(-c2ccc(Br)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6b21c13c0f3b44b3bddb7e6cd4e61e8f
BrP(Br)(c1ccccc1)(c1ccccc1)c1ccccc1.OCc1ccc(-c2ccc(Br)cc2)cc1>>BrCc1ccc(-c2ccc(Br)cc2)cc1
BrC1=CC=C(C=C1)C1=CC=C(C=C1)CO.BrP(C1=CC=CC=C1)(C1=CC=CC=C1)(C1=CC=CC=C1)Br>>BrC1=CC=C(C=C1)C1=CC=C(C=C1)CBr
BrP(c1ccccc1)(c1ccccc1)(c1ccccc1)[Br:1].O[CH2:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([Br:11])[cH:12][cH:13]2)[cH:14][cH:15]1>>[Br:1][CH2:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([Br:11])[cH:12][cH:13]2)[cH:14][cH:15]1
BrP(Br)(c1ccccc1)(c1ccccc1)c1ccccc1.OCc1ccc(-c2ccc(Br)cc2)cc1
BrCc1ccc(-c2ccc(Br)cc2)cc1
null
null
O.C(Cl)Cl
Functional Group Interconversion
OtherReaction
8872f2fae3cc46ec19a3bd8f9f9484c21a537e6d42617740a795333c61c3afc4
cbf41c7cf9fe6b47a243b1674d74ed5bf46a151f7f3a71d206e23176e158facf
c1ccc(-c2ccccc2)cc1
Br-P(-[Br;H0;D1;+0:1])(-c1:c:c:c:c:c:1)(-c1:c:c:c:c:c:1)-c1:c:c:c:c:c:1.O-[CH2;D2;+0:2]-[c:3](:[c:4]):[c:5]>>[Br;H0;D1;+0:1]-[CH2;D2;+0:2]-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
A solution of (4′-bromo-biphenyl-4-yl)-methanol, 7.01 g (27.9 mmol) and dibromo-triphenylphosphorane 11.8 g (27.9 mmol) in 150 mL of methylene chloride stirred at room temperature for 2 h. The solution was diluted with 100 mL of water and extracted with 2×200 mL portions of diethyl ether. The organic layers were combin...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Primary halide
c1ccccc1.c1ccccc1.c1ccccc1
null
c1ccccc1.c1ccccc1
HBr
O.C(Cl)Cl
null
null
BrP(Br)(c1ccccc1)(c1ccccc1)c1ccccc1.OCc1ccc(-c2ccc(Br)cc2)cc1>O.C(Cl)Cl>BrCc1ccc(-c2ccc(Br)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2a5c271ada4a460a91ac4613c6188126
BrCc1ccc(-c2ccc(Br)cc2)cc1.COC(=O)[C@H](CS)NC(=O)OC(C)(C)C>>COC(=O)C(CSCc1ccc(-c2ccc(Br)cc2)cc1)NC(=O)OC(C)(C)C
BrC1=CC=C(C=C1)C1=CC=C(C=C1)CBr.COC([C@@H](NC(=O)OC(C)(C)C)CS)=O.C([O-])([O-])=O.[Cs+].[Cs+].CN(C=O)C>>COC(C(CSCC1=CC=C(C=C1)C1=CC=C(C=C1)Br)NC(=O)OC(C)(C)C)=O
Br[CH2:8][c:9]1[cH:10][cH:11][c:12](-[c:13]2[cH:14][cH:15][c:16]([Br:17])[cH:18][cH:19]2)[cH:20][cH:21]1.[CH3:1][O:2][C:3](=[O:4])[C@H:5]([CH2:6][SH:7])[NH:22][C:23](=[O:24])[O:25][C:26]([CH3:27])([CH3:28])[CH3:29]>>[CH3:1][O:2][C:3](=[O:4])[CH:5]([CH2:6][S:7][CH2:8][c:9]1[cH:10][cH:11][c:12](-[c:13]2[cH:14][cH:15][c:1...
BrCc1ccc(-c2ccc(Br)cc2)cc1.COC(=O)[C@H](CS)NC(=O)OC(C)(C)C
COC(=O)C(CSCc1ccc(-c2ccc(Br)cc2)cc1)NC(=O)OC(C)(C)C
null
null
O
Heteroatom Alkylation and Arylation
thioether_nucl_sub
77cd742b5ba20df0e225494f6e5f3d958ee82ce9a1b16fd99a2d9f8350b4fdc8
b05f7dda7dad719ae1868a84c33eeaf5bf649036fc64173cf4774a5eb4d70181
c1ccc(-c2ccccc2)cc1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[#8:5]-[C:6](=[O;D1;H0:7])-[C:8]-[C:9]-[SH;D1;+0:10]>>[#8:5]-[C:6](=[O;D1;H0:7])-[C:8]-[C:9]-[S;H0;D2;+0:10]-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
4
HOUR
A mixture of 4′-Bromo-4-bromomethyl-biphenyl, 9.1 g (27.9 mmol), N-(tert-Butoxy-carbonyl)-L-cysteine methyl ester, 5.74 mL (27.9 mmol), cesium carbonate, 18.2 g (55.8 mmol), and 100 mL of N,N-dimethylformamide was stirred at room temperature for 4 h. The mixture was diluted with 200 mL of water and extracted with 2×200...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aliphatic thiol
Monosulfide
null
null
c1ccccc1.c1ccccc1
HBr
O
null
4
BrCc1ccc(-c2ccc(Br)cc2)cc1.COC(=O)[C@H](CS)NC(=O)OC(C)(C)C>O>COC(=O)C(CSCc1ccc(-c2ccc(Br)cc2)cc1)NC(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-924209de829f46698e0c5472ddea0acc
COC(=O)C(CSCc1ccc(-c2ccc(Br)cc2)cc1)NC(=O)OC(C)(C)C.OB(O)c1ccc2c(c1)OCO2>>COC(=O)C(N)(CSCc1ccc(-c2ccc(-c3ccc4c(c3)OCO4)cc2)cc1)C(=O)OC(C)(C)C
C(=O)([O-])[O-].[Na+].[Na+].C(C)O.C1(=CC=CC=C1)C.COC(C(CSCC1=CC=C(C=C1)C1=CC=C(C=C1)Br)NC(=O)OC(C)(C)C)=O.C1OC=2C=C(C=CC2O1)B(O)O>>COC(C(CSCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC2=C(OCO2)C=C1)(C(=O)OC(C)(C)C)N)=O
Br[c:17]1[cH:16][cH:15][c:14](-[c:13]2[cH:12][cH:11][c:10]([CH2:9][S:8][CH2:7][CH:5]([C:3]([O:2][CH3:1])=[O:4])[NH:6][C:31](=[O:32])[O:33][C:34]([CH3:35])([CH3:36])[CH3:37])[cH:30][cH:29]2)[cH:28][cH:27]1.OB(O)[c:18]1[cH:19][cH:20][c:21]2[c:22]([cH:23]1)[O:24][CH2:25][O:26]2>>[CH3:1][O:2][C:3](=[O:4])[C:5]([NH2:6])([CH...
COC(=O)C(CSCc1ccc(-c2ccc(Br)cc2)cc1)NC(=O)OC(C)(C)C.OB(O)c1ccc2c(c1)OCO2
COC(=O)C(N)(CSCc1ccc(-c2ccc(-c3ccc4c(c3)OCO4)cc2)cc1)C(=O)OC(C)(C)C
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
C(C)(=O)OCC
C-C Coupling
OtherReaction
8bfdeabe353177261302af58ff5d125f7cc327422930bad1cf6fd6e991251f27
e5c3d9302fdfa5543f6fae69ac941917f16ef75f0b4c9bd17dbd8e8ddd91a4bb
c1ccc(-c2ccc(-c3ccc4c(c3)OCO4)cc2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[#16:6]-[C:7]-[CH;D3;+0:8](-[NH;D2;+0:9]-[C;H0;D3;+0:10](=[O;D1;H0:11])-[#8:12]-[C:13](-[C;D1;H3:14])(-[C;D1;H3:15])-[C;D1;H3:16])-[C:17](=[O;D1;H0:18])-[#8:19]-[C;D1;H3:20].O-B(-O)-[c;H0;D3;+0:21](:[c:22]:[c:23]):[c:24]:[c:25]-[#8:26]>>[#16:6]-[C:7]-[C;H0;D4;+0:8](-[NH2;D1;+...
null
[]
80
CELSIUS
null
null
A mixture of 3-(4′-bromobiphenyl-4-ylmethylsulfanyl)-2-tert-butoxycarbonylamino-propionic acid methyl ester, 0.26 g (0.54 mmol), 3,4-methylenedioxyphenylboronic acid, 90 mg (0.54 mmol), Pd(PPh3)4, 63 mg (0.054 mmol), in 5 mL of toluene and 3 mL of ethanol was heated to obtain a clear solution. To the solution was added...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Carbamic ester.Ester.Ether.Boronic acid
Ester.Ester.Primary amine.Boc
c1ccccc1.c1ccc2c(c1)OCO2
c1ccccc1.c1ccc2c(c1)OCO2
c1ccccc1.c1ccccc1.c1ccc2c(c1)OCO2
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C(C)(=O)OCC
80
null
COC(=O)C(CSCc1ccc(-c2ccc(Br)cc2)cc1)NC(=O)OC(C)(C)C.OB(O)c1ccc2c(c1)OCO2>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C(C)(=O)OCC>COC(=O)C(N)(CSCc1ccc(-c2ccc(-c3ccc4c(c3)OCO4)cc2)cc1)C(=O)OC(C)(...
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3e0ced95fa914006b48b49eb33157ff9
COC(=O)C(CS)NC(=O)OC(C)(C)C.O=[N+]([O-])c1ccc(CBr)cc1>>COC(=O)[C@H](CSCc1ccc(N)cc1)NC(=O)OC(C)(C)C
BrCC1=CC=C(C=C1)[N+](=O)[O-].C([O-])([O-])=O.[Cs+].[Cs+].COC(C(CS)NC(=O)OC(C)(C)C)=O.C(C)(=O)OCC>>COC([C@H](CSCC1=CC=C(C=C1)N)NC(=O)OC(C)(C)C)=O
[CH3:1][O:2][C:3](=[O:4])[CH:5]([CH2:6][SH:7])[NH:16][C:17](=[O:18])[O:19][C:20]([CH3:21])([CH3:22])[CH3:23].O=[N+:13]([O-])[c:12]1[cH:11][cH:10][c:9]([CH2:8]Br)[cH:15][cH:14]1>>[CH3:1][O:2][C:3](=[O:4])[C@H:5]([CH2:6][S:7][CH2:8][c:9]1[cH:10][cH:11][c:12]([NH2:13])[cH:14][cH:15]1)[NH:16][C:17](=[O:18])[O:19][C:20]([CH...
COC(=O)C(CS)NC(=O)OC(C)(C)C.O=[N+]([O-])c1ccc(CBr)cc1
COC(=O)[C@H](CSCc1ccc(N)cc1)NC(=O)OC(C)(C)C
null
null
CCCCCCC.CN(C)C=O
Functional Group Interconversion
OtherReaction
553deca63c3a8c4d19c0ad505165c3556b3a45eedc28fd1d37d79d0ef5f89b4b
e4ebb23b210d1b6420aef2681cd46eddaa6b419e415077c98e81572b75a5dacb
c1ccccc1
Br-[CH2;D2;+0:1]-[c:2]1:[c:3]:[c:4]:[c:5](-[N+;H0;D3:6](=O)-[O-]):[c:7]:[c:8]:1.[#8:9]-[C:10](=[O;D1;H0:11])-[C:12]-[C:13]-[SH;D1;+0:14]>>[#8:9]-[C:10](=[O;D1;H0:11])-[C:12]-[C:13]-[S;H0;D2;+0:14]-[CH2;D2;+0:1]-[c:2]1:[c:3]:[c:4]:[c:5](-[NH2;D1;+0:6]):[c:7]:[c:8]:1
null
[]
null
null
null
null
A mixture of 1-bromomethyl-4-nitro-benzene (2.15 g, 9.95 mmol), cesium carbonate (6.49 g, 19.9 mmol) and 2-tert-butoxycarbonylamino-3-mercapto-propionic acid methyl ester (2.46 g, 10.5 mmol) in DMF (25 mL) was stirred at room temperature. Upon completion of the reaction (TLC control: 30% ethyl acetate in heptane), the ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Nitro group.Aliphatic thiol
Primary amine.Monosulfide
null
null
c1ccccc1
Br-
CCCCCCC.CN(C)C=O
null
null
COC(=O)C(CS)NC(=O)OC(C)(C)C.O=[N+]([O-])c1ccc(CBr)cc1>CCCCCCC.CN(C)C=O>COC(=O)[C@H](CSCc1ccc(N)cc1)NC(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d1c8218e96c0429f89ef8054ddc0d591
COC(=O)[C@H](CSCc1ccc([N+](=O)[O-])cc1)NC(=O)OC(C)(C)C>>COC(=O)[C@H](CSCc1ccc(N)cc1)NC(=O)OC(C)(C)C
COC([C@H](CSCC1=CC=C(C=C1)[N+](=O)[O-])NC(=O)OC(C)(C)C)=O.[Sn](Cl)Cl>>COC([C@H](CSCC1=CC=C(C=C1)N)NC(=O)OC(C)(C)C)=O
O=[N+:13]([O-])[c:12]1[cH:11][cH:10][c:9]([CH2:8][S:7][CH2:6][C@@H:5]([C:3]([O:2][CH3:1])=[O:4])[NH:16][C:17](=[O:18])[O:19][C:20]([CH3:21])([CH3:22])[CH3:23])[cH:15][cH:14]1>>[CH3:1][O:2][C:3](=[O:4])[C@H:5]([CH2:6][S:7][CH2:8][c:9]1[cH:10][cH:11][c:12]([NH2:13])[cH:14][cH:15]1)[NH:16][C:17](=[O:18])[O:19][C:20]([CH3:...
COC(=O)[C@H](CSCc1ccc([N+](=O)[O-])cc1)NC(=O)OC(C)(C)C
COC(=O)[C@H](CSCc1ccc(N)cc1)NC(=O)OC(C)(C)C
null
null
ClCCl.CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccccc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
50
CELSIUS
null
null
A mixture of (2R)-methyl-2-tert-butoxycarbonylamino-3-(4-nitro-benzylsulfanyl)-propionate (3.75 g, 10.1 mmol) and tin (II) chloride (5.76 g, 30.0 mmol) in methanol (50 mL) was stirred at 50° C. Upon completion (TLC: 5% methanol in dichloromethane), the mixture was cooled to room temperature, quenched with saturated pot...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1
Other
ClCCl.CO
50
null
COC(=O)[C@H](CSCc1ccc([N+](=O)[O-])cc1)NC(=O)OC(C)(C)C>ClCCl.CO>COC(=O)[C@H](CSCc1ccc(N)cc1)NC(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b9bc9c368d9240b2aab2a92d59f507ce
CCOC(=O)Cn1ccc2ccccc21>>O=C(O)Cn1ccc2ccccc21
N1C=CC2=CC=CC=C12.[H-].[Na+].Cl.C(C)OC(CN1C=CC2=CC=CC=C12)=O.[OH-].[Na+].C(C)OC(CBr)=O>>N1(C=CC2=CC=CC=C12)CC(=O)O
CC[O:3][C:2](=[O:1])[CH2:4][n:5]1[cH:6][cH:7][c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]12>>[O:1]=[C:2]([OH:3])[CH2:4][n:5]1[cH:6][cH:7][c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]12
CCOC(=O)Cn1ccc2ccccc21
O=C(O)Cn1ccc2ccccc21
null
null
ClCCl.CO.CN(C)C=O.C1CCOC1
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc2[nH]ccc2c1
C-C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
null
[]
70
CELSIUS
null
null
1H-indole (5.0 g, 42.7 mmol) in anhydrous DMF (10 mL) was added to a suspension of sodium hydride (1.13 g, 46.9 mmol) in anhydrous DMF (20 mL) in a flame dried flask at 0° C. stirred under nitrogen atmosphere. Fifteen minutes after gas evolution had ceased, bromo-acetic acid ethyl ester (5.7 mL, 51.2 mmol) was added an...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccc2[nH]ccc2c1
Other
ClCCl.CO.CN(C)C=O.C1CCOC1
70
null
CCOC(=O)Cn1ccc2ccccc21>ClCCl.CO.CN(C)C=O.C1CCOC1>O=C(O)Cn1ccc2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ccde56c91db340b7b0fea8969f019ce6
COC(=O)[C@H](CSCc1ccc(N)cc1)NC(=O)OC(C)(C)C.O=C(O)Cn1ccc2ccccc21>>CC(C)(C)OC(=O)N[C@@H](CSCc1ccc(NC(=O)Cn2ccc3ccccc32)cc1)C(=O)O
[OH-].[Na+].Cl.COC([C@H](CSCC1=CC=C(C=C1)NC(CN1C=CC2=CC=CC=C12)=O)NC(=O)OC(C)(C)C)=O.N1(C=CC2=CC=CC=C12)CC(=O)O.COC([C@H](CSCC1=CC=C(C=C1)N)NC(=O)OC(C)(C)C)=O.C(CCl)Cl.C(C)N(CC)CC>>C(C)(C)(C)OC(=O)N[C@H](C(=O)O)CSCC1=CC=C(C=C1)NC(CN1C=CC2=CC=CC=C12)=O
C[O:34][C:32]([C@@H:9]([NH:8][C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[CH2:10][S:11][CH2:12][c:13]1[cH:14][cH:15][c:16]([NH2:17])[cH:30][cH:31]1)=[O:33].O[C:18](=[O:19])[CH2:20][n:21]1[cH:22][cH:23][c:24]2[cH:25][cH:26][cH:27][cH:28][c:29]12>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[NH:8][C@@H:9]([CH2:1...
COC(=O)[C@H](CSCc1ccc(N)cc1)NC(=O)OC(C)(C)C.O=C(O)Cn1ccc2ccccc21
CC(C)(C)OC(=O)N[C@@H](CSCc1ccc(NC(=O)Cn2ccc3ccccc32)cc1)C(=O)O
null
CN(C)C=1C=CN=CC1
C(C)(=O)OCC.CCCCCCC.CO.C(Cl)Cl.ClCCl.C1CCOC1
Acylation
OtherReaction
2f4be8b14ede2d52c920d439e5f741d97aa4249f4c57807152c62994aca84307
87a69d5ad38be49e96448ab38c6e7071a2232ada5542b6b62a2f1e1b1e6e076f
O=C(Cn1ccc2ccccc21)Nc1ccccc1
C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4].[NH2;D1;+0:5]-[c:6](:[c:7]):[c:8].O-[C;H0;D3;+0:9](=[O;D1;H0:10])-[C:11]-[#7;a:12]>>[#7;a:12]-[C:11]-[C;H0;D3;+0:9](=[O;D1;H0:10])-[NH;D2;+0:5]-[c:6](:[c:7]):[c:8].[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
null
[]
null
null
null
null
A solution of indol-1-yl-acetic acid (1.25 g, 7.14 mmol), (2R)-3-(4-amino-benzylsulfanyl)-2-tert-butoxycarbonylamino-propionic acid methyl ester (2.67 g, 7.85 mmol), EDC (1.71 g, 8.93 mmol), triethylamine (2.48 mL, 17.85 mmol) and DMAP (87 mg, 0.714 mmol) in DCM (50 mL) was stirred at ambient temperature. Upon completi...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Ester.Primary amine
Carboxylic acid.Secondary amide
null
null
c1ccccc1.c1ccc2[nH]ccc2c1
HO-
CN(C)C=1C=CN=CC1.C(C)(=O)OCC.CCCCCCC.CO.C(Cl)Cl.ClCCl.C1CCOC1
null
null
COC(=O)[C@H](CSCc1ccc(N)cc1)NC(=O)OC(C)(C)C.O=C(O)Cn1ccc2ccccc21>CN(C)C=1C=CN=CC1.C(C)(=O)OCC.CCCCCCC.CO.C(Cl)Cl.ClCCl.C1CCOC1>CC(C)(C)OC(=O)N[C@@H](CSCc1ccc(NC(=O)Cn2ccc3ccccc32)cc1)C(=O)O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f5ab36560acc4cb5812d92c3f885bfc0
CC(C)(C)OC(=O)N[C@@H](CSCc1ccc(NC(=O)Cn2ccc3cc(F)ccc32)cc1)C(=O)O>>CC(C)(C)OC(=O)N[C@@H](CS(=O)Cc1ccc(NC(=O)Cn2ccc3cc(F)ccc32)cc1)C(=O)O
CO.C(C)(C)(C)OC(=O)N[C@H](C(=O)O)CSCC1=CC=C(C=C1)NC(CN1C=CC2=CC(=CC=C12)F)=O.B1(OO1)[O-].O.O.O.O.[Na+]>>C(C)(C)(C)OC(=O)N[C@H](C(=O)O)CS(=O)CC1=CC=C(C=C1)NC(CN1C=CC2=CC(=CC=C12)F)=O
[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[NH:8][C@@H:9]([CH2:10][S:11][CH2:13][c:14]1[cH:15][cH:16][c:17]([NH:18][C:19](=[O:20])[CH2:21][n:22]2[cH:23][cH:24][c:25]3[cH:26][c:27]([F:28])[cH:29][cH:30][c:31]23)[cH:32][cH:33]1)[C:34](=[O:35])[OH:36]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[NH:8][C@@H:9]([C...
CC(C)(C)OC(=O)N[C@@H](CSCc1ccc(NC(=O)Cn2ccc3cc(F)ccc32)cc1)C(=O)O
CC(C)(C)OC(=O)N[C@@H](CS(=O)Cc1ccc(NC(=O)Cn2ccc3cc(F)ccc32)cc1)C(=O)O
null
null
ClCCl.C(C)(=O)O.C(C)(=O)OCC
Oxidation
Sulfanyl to sulfinyl
9edfaf6d72a81452ea8e3a1cdcb10a58409fff36608e97019e7273998b3d5373
f5f6bb6ca76a2267cd589767b4d67e7a17ab1ac383eeb6143dcd5d92e00e1b6a
O=C(Cn1ccc2ccccc21)Nc1ccccc1
[O;D1;H0:1]=[C:2](-[O;D1;H1:3])-[C:4]-[C:5]-[S;H0;D2;+0:6]-[C:7]-[c:8]>>[O;D1;H0:9]=[S;H0;D3;+0:6](-[C:5]-[C:4]-[C:2](=[O;D1;H0:1])-[O;D1;H1:3])-[C:7]-[c:8]
null
[]
null
null
null
null
To a stirred solution of (2R)-2-tert-butoxycarbonylamino-3-{4-[2-(5-fluoro-indol-1-yl)-acetylamino]-benzylsulfanyl}-propionic acid (460 mg, 0.917 mmol) in acetic acid (20 mL) was added sodium perborate tetrahydrate (148 mg, 0.963 mmol). This solution was stirred at 40° C. until complete (TLC: 20% methanol in dichlorome...
10.6084/m9.figshare.5104873.v1
null
Monosulfide
Sulfoxide
null
null
c1ccccc1.c1ccc2[nH]ccc2c1
null
ClCCl.C(C)(=O)O.C(C)(=O)OCC
null
null
CC(C)(C)OC(=O)N[C@@H](CSCc1ccc(NC(=O)Cn2ccc3cc(F)ccc32)cc1)C(=O)O>ClCCl.C(C)(=O)O.C(C)(=O)OCC>CC(C)(C)OC(=O)N[C@@H](CS(=O)Cc1ccc(NC(=O)Cn2ccc3cc(F)ccc32)cc1)C(=O)O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-58f58401393a45d59b85a43a7bd85fc0
CCCCc1cc2ccccc2o1.O=C(Cl)c1ccc(Br)cc1>>CCCCc1oc2ccccc2c1C(=O)c1ccc(Br)cc1
C(CCC)C=1OC2=C(C1)C=CC=C2.BrC1=CC=C(C(=O)Cl)C=C1.[Al+3].[Cl-].[Cl-].[Cl-]>>BrC1=CC=C(C=C1)C(=O)C1=C(OC2=C1C=CC=C2)CCCC
[CH3:1][CH2:2][CH2:3][CH2:4][c:5]1[o:6][c:7]2[cH:8][cH:9][cH:10][cH:11][c:12]2[cH:13]1.Cl[C:14](=[O:15])[c:16]1[cH:17][cH:18][c:19]([Br:20])[cH:21][cH:22]1>>[CH3:1][CH2:2][CH2:3][CH2:4][c:5]1[o:6][c:7]2[cH:8][cH:9][cH:10][cH:11][c:12]2[c:13]1[C:14](=[O:15])[c:16]1[cH:17][cH:18][c:19]([Br:20])[cH:21][cH:22]1
CCCCc1cc2ccccc2o1.O=C(Cl)c1ccc(Br)cc1
CCCCc1oc2ccccc2c1C(=O)c1ccc(Br)cc1
null
null
ClCCl
C-C Coupling
Friedel-Crafts acylation
b92ea6a688e6ba35d387a21fbedc1e5690fb4da234146ba469a67b2fc1ec6714
fe2a4a0dfbb5b71b9a065e092364c64b22b4eb1ad4d6ba2a1e8edc9d31fce3e4
O=C(c1ccccc1)c1coc2ccccc12
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C:6]-[c:7]1:[#8;a:8]:[c:9](:[c:10]):[c:11](:[c:12]):[cH;D2;+0:13]:1>>[C:6]-[c:7]1:[#8;a:8]:[c:9](:[c:10]):[c:11](:[c:12]):[c;H0;D3;+0:13]:1-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
36
[{"value": 36.0, "product": "BrC1=CC=C(C=C1)C(=O)C1=C(OC2=C1C=CC=C2)CCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 35.8, "product": "BrC1=CC=C(C=C1)C(=O)C1=C(OC2=C1C=CC=C2)CCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
A solution of 2-n-butylbenzofurane (19.8 g, 114 mmol) and 4-bromobenzoyl chloride (25.0 g, 114 mmol) in dry dichloromethane (300 mL, 0.4 M) was cooled to 0° C. and treated with AlCl3 (16.6 g, 1.1 equiv., 125.4 mmol) in 3 portions. After the additions were complete, the solution was stirred for 3 h and carefully added t...
10.6084/m9.figshare.5104873.v1
null
Acyl halide
Ketone
c1ccc2occc2c1
c1ccc2occc2c1
c1ccc2occc2c1.c1ccccc1
HCl
ClCCl
null
3
CCCCc1cc2ccccc2o1.O=C(Cl)c1ccc(Br)cc1>ClCCl>CCCCc1oc2ccccc2c1C(=O)c1ccc(Br)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c4268f2ef6eb48fa95d250d115fed018
CCCCc1oc2ccccc2c1Cc1ccc(-c2ccc(OCCCc3ccccc3)c([N+](=O)[O-])c2)cc1>>CCCCc1oc2ccccc2c1Cc1ccc(-c2ccc(OCCCc3ccccc3)c(N)c2)cc1
C(CCC)C=1OC2=C(C1CC1=CC=C(C=C1)C1=CC(=C(C=C1)OCCCC1=CC=CC=C1)[N+](=O)[O-])C=CC=C2>>C(CCC)C=1OC2=C(C1CC1=CC=C(C=C1)C1=CC(=C(C=C1)OCCCC1=CC=CC=C1)N)C=CC=C2
O=[N+:34]([O-])[c:33]1[c:22]([O:23][CH2:24][CH2:25][CH2:26][c:27]2[cH:28][cH:29][cH:30][cH:31][cH:32]2)[cH:21][cH:20][c:19](-[c:18]2[cH:17][cH:16][c:15]([CH2:14][c:13]3[c:5]([CH2:4][CH2:3][CH2:2][CH3:1])[o:6][c:7]4[cH:8][cH:9][cH:10][cH:11][c:12]43)[cH:37][cH:36]2)[cH:35]1>>[CH3:1][CH2:2][CH2:3][CH2:4][c:5]1[o:6][c:7]2...
CCCCc1oc2ccccc2c1Cc1ccc(-c2ccc(OCCCc3ccccc3)c([N+](=O)[O-])c2)cc1
CCCCc1oc2ccccc2c1Cc1ccc(-c2ccc(OCCCc3ccccc3)c(N)c2)cc1
null
[Fe]
C(C)(=O)O.C(C)O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc(CCCOc2ccc(-c3ccc(Cc4coc5ccccc45)cc3)cc2)cc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
29
[{"value": 29.0, "product": "C(CCC)C=1OC2=C(C1CC1=CC=C(C=C1)C1=CC(=C(C=C1)OCCCC1=CC=CC=C1)N)C=CC=C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 28.2, "product": "C(CCC)C=1OC2=C(C1CC1=CC=C(C=C1)C1=CC(=C(C=C1)OCCCC1=CC=CC=C1)N)C=CC=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
120
CELSIUS
null
null
A solution of 2-butyl-3-[3′-nitro-4′-(3-phenyl-propoxy)-biphenyl-4-ylmethyl]-benzofuran (53 mg, 0.105 mmol) in ethanol (1 mL) and acetic acid (1 mL) was treated with Fe (26.4 mg, 4.5 equiv., 0.472 mmol) and heated to 120° C. for 3 h. After cooling to room temperature, the solution was poured into a 20% aq NaOH/ice wate...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccc2occc2c1.c1ccccc1.c1ccccc1.c1ccccc1
Other
[Fe].C(C)(=O)O.C(C)O
120
null
CCCCc1oc2ccccc2c1Cc1ccc(-c2ccc(OCCCc3ccccc3)c([N+](=O)[O-])c2)cc1>[Fe].C(C)(=O)O.C(C)O>CCCCc1oc2ccccc2c1Cc1ccc(-c2ccc(OCCCc3ccccc3)c(N)c2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-08c148bcbf344169864e17a15718c071
CCCCc1oc2ccccc2c1Cc1ccc(-c2ccc(OCCCc3ccccc3)c(N)c2)cc1.CCOC(=O)C(=O)Cl>>CCCCc1oc2ccccc2c1Cc1ccc(-c2ccc(OCCCc3ccccc3)c(NC(=O)C(=O)OCC)c2)cc1
C(CCC)C=1OC2=C(C1CC1=CC=C(C=C1)C1=CC(=C(C=C1)OCCCC1=CC=CC=C1)N)C=CC=C2.C(C)(C)N(CC)C(C)C.ClC(C(=O)OCC)=O>>C(C)OC(C(=O)NC=1C=C(C=CC1OCCCC1=CC=CC=C1)C1=CC=C(C=C1)CC1=C(OC2=C1C=CC=C2)CCCC)=O
[CH3:1][CH2:2][CH2:3][CH2:4][c:5]1[o:6][c:7]2[cH:8][cH:9][cH:10][cH:11][c:12]2[c:13]1[CH2:14][c:15]1[cH:16][cH:17][c:18](-[c:19]2[cH:20][cH:21][c:22]([O:23][CH2:24][CH2:25][CH2:26][c:27]3[cH:28][cH:29][cH:30][cH:31][cH:32]3)[c:33]([NH2:34])[cH:42]2)[cH:43][cH:44]1.Cl[C:35](=[O:36])[C:37](=[O:38])[O:39][CH2:40][CH3:41]>...
CCCCc1oc2ccccc2c1Cc1ccc(-c2ccc(OCCCc3ccccc3)c(N)c2)cc1.CCOC(=O)C(=O)Cl
CCCCc1oc2ccccc2c1Cc1ccc(-c2ccc(OCCCc3ccccc3)c(NC(=O)C(=O)OCC)c2)cc1
null
null
ClCCl.O
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
a0f509c51b80cfca9aa6355468af6f3d901b4a3653602f32ee5994157ced49f8
41a2c91a94881e86389ce33bb44cfd1f3b3dc1b8c84cd64ddc8a356ca8fd86c3
c1ccc(CCCOc2ccc(-c3ccc(Cc4coc5ccccc45)cc3)cc2)cc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](=[O;D1;H0:4])-[#8:5]-[C:6].[NH2;D1;+0:7]-[c:8](:[c:9]):[c:10]>>[C:6]-[#8:5]-[C:3](=[O;D1;H0:4])-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:7]-[c:8](:[c:9]):[c:10]
77.1
[{"value": 77.0, "product": "C(C)OC(C(=O)NC=1C=C(C=CC1OCCCC1=CC=CC=C1)C1=CC=C(C=C1)CC1=C(OC2=C1C=CC=C2)CCCC)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 77.1, "product": "C(C)OC(C(=O)NC=1C=C(C=CC1OCCCC1=CC=CC=C1)C1=CC=C(C=C1)CC1=C(OC2=C1C=CC=C2)CCCC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desir...
null
null
2
HOUR
A solution of 4′-(2-butyl-benzofuran-3-ylmethyl)-4-(3-phenyl-propoxy)-biphenyl-3-ylamine (129 mg, 0.264 mmol) and diisopropylethylamine (0.115 mL, 2.5 equiv., 0.66 mmol) in dichloromethane (5 mL) was treated with a solution of ethyl chlorooxoacetate (44 mg, 1.2 equiv., 0.317 mmol) in dichloromethane (1 mL). After stirr...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Ester.Primary amine
Ester.Secondary amide
null
null
c1ccc2occc2c1.c1ccccc1.c1ccccc1.c1ccccc1
HCl
ClCCl.O
null
2
CCCCc1oc2ccccc2c1Cc1ccc(-c2ccc(OCCCc3ccccc3)c(N)c2)cc1.CCOC(=O)C(=O)Cl>ClCCl.O>CCCCc1oc2ccccc2c1Cc1ccc(-c2ccc(OCCCc3ccccc3)c(NC(=O)C(=O)OCC)c2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-66a338ee4d88413c8f774dee44584a97
CCCCc1oc2ccccc2c1Cc1ccc(-c2ccc(OCCCc3ccccc3)c(NC(=O)C(=O)OCC)c2)cc1>>CCCCc1oc2ccccc2c1Cc1ccc(-c2ccc(OCCCc3ccccc3)c(NC(=O)C(=O)O)c2)cc1
Cl.C(C)OC(C(=O)NC=1C=C(C=CC1OCCCC1=CC=CC=C1)C1=CC=C(C=C1)CC1=C(OC2=C1C=CC=C2)CCCC)=O.[OH-].[Na+]>>C(CCC)C=1OC2=C(C1CC1=CC=C(C=C1)C1=CC(=C(C=C1)OCCCC1=CC=CC=C1)NC(C(=O)O)=O)C=CC=C2
CC[O:39][C:37]([C:35]([NH:34][c:33]1[c:22]([O:23][CH2:24][CH2:25][CH2:26][c:27]2[cH:28][cH:29][cH:30][cH:31][cH:32]2)[cH:21][cH:20][c:19](-[c:18]2[cH:17][cH:16][c:15]([CH2:14][c:13]3[c:5]([CH2:4][CH2:3][CH2:2][CH3:1])[o:6][c:7]4[cH:8][cH:9][cH:10][cH:11][c:12]43)[cH:42][cH:41]2)[cH:40]1)=[O:36])=[O:38]>>[CH3:1][CH2:2][...
CCCCc1oc2ccccc2c1Cc1ccc(-c2ccc(OCCCc3ccccc3)c(NC(=O)C(=O)OCC)c2)cc1
CCCCc1oc2ccccc2c1Cc1ccc(-c2ccc(OCCCc3ccccc3)c(NC(=O)C(=O)O)c2)cc1
null
null
C(C)O
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(CCCOc2ccc(-c3ccc(Cc4coc5ccccc45)cc3)cc2)cc1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[C:4](=[O;D1;H0:5])-[#7:6]-[c:7]>>[O;D1;H0:5]=[C:4](-[#7:6]-[c:7])-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
28
[{"value": 28.0, "product": "C(CCC)C=1OC2=C(C1CC1=CC=C(C=C1)C1=CC(=C(C=C1)OCCCC1=CC=CC=C1)NC(C(=O)O)=O)C=CC=C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 27.9, "product": "C(CCC)C=1OC2=C(C1CC1=CC=C(C=C1)C1=CC(=C(C=C1)OCCCC1=CC=CC=C1)NC(C(=O)O)=O)C=CC=C2", "details": "CALCULATEDPERCENTYIELD", "is_desir...
null
null
null
null
A solution of N-[4′-(2-butyl-benzofuran-3-ylmethyl)-4-(3-phenyl-propoxy)-biphenyl-3-yl]-oxalamic acid ethyl ester (120 mg, 0.204 mmol) in ethanol (3 mL) was treated with aq 1 N NaOH (0.3 mL, 1.5 equiv., 0.306 mmol) and stirred at room temperature. After stirring 1 h, the solution was acidified to pH<4 with 10% HCl, con...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccc2occc2c1.c1ccccc1.c1ccccc1.c1ccccc1
Other
C(C)O
null
null
CCCCc1oc2ccccc2c1Cc1ccc(-c2ccc(OCCCc3ccccc3)c(NC(=O)C(=O)OCC)c2)cc1>C(C)O>CCCCc1oc2ccccc2c1Cc1ccc(-c2ccc(OCCCc3ccccc3)c(NC(=O)C(=O)O)c2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-101023113fe040809a5c82f0e36ff349
C[Si](C)(C)c1ccc(Br)cc1.OB(O)c1cccc2c1oc1ccccc12>>C[Si](C)(C)c1ccc(-c2cccc3c2oc2ccccc23)cc1
C1=CC=C(C=2OC3=C(C21)C=CC=C3)B(O)O.BrC1=CC=C(C=C1)[Si](C)(C)C.C(=O)([O-])[O-].[K+].[K+]>>C1=CC=C(C=2OC3=C(C21)C=CC=C3)C3=CC=C(C=C3)[Si](C)(C)C
Br[c:8]1[cH:7][cH:6][c:5]([Si:2]([CH3:1])([CH3:3])[CH3:4])[cH:23][cH:22]1.OB(O)[c:9]1[cH:10][cH:11][cH:12][c:13]2[c:14]1[o:15][c:16]1[cH:17][cH:18][cH:19][cH:20][c:21]21>>[CH3:1][Si:2]([CH3:3])([CH3:4])[c:5]1[cH:6][cH:7][c:8](-[c:9]2[cH:10][cH:11][cH:12][c:13]3[c:14]2[o:15][c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]32)[c...
C[Si](C)(C)c1ccc(Br)cc1.OB(O)c1cccc2c1oc1ccccc12
C[Si](C)(C)c1ccc(-c2cccc3c2oc2ccccc23)cc1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.C1(=CC=CC=C1)C.C(C)O
C-C Coupling
Suzuki coupling with boronic acids
a34fd3f8e97b635d120df300575865eab1505627afd99c75ec2034d5929796bd
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2cccc3c2oc2ccccc23)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9](:[c:10]):[#8;a:11]:[c:12]>>[c:8]:[c:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9](:[c:10]):[#8;a:11]:[c:12]
96.8
[{"value": 96.0, "product": "C1=CC=C(C=2OC3=C(C21)C=CC=C3)C3=CC=C(C=C3)[Si](C)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 96.8, "product": "C1=CC=C(C=2OC3=C(C21)C=CC=C3)C3=CC=C(C=C3)[Si](C)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
null
null
A solution of dibenzofuran-4-yl-boronic acid (20.0 g, 94.3 mmol), (4-bromo-phenyl)-trimethyl-silane (21.62 g, 94.3 mmol), K2CO3 (39.1 g, 3 equiv., 283 mmol) in toluene (100 mL), ethanol (60 mL) and water (30 mL) was purged with nitrogen for 5 min (bubbled into solution) and treated with Pd(PPh3)4 (3.59 g, 2.9 mmol). Af...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccc2c(c1)oc1ccccc12
c1ccccc1.c1ccc2c(c1)oc1ccccc12
c1ccccc1.c1ccc2c(c1)oc1ccccc12
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.C1(=CC=CC=C1)C.C(C)O
80
null
C[Si](C)(C)c1ccc(Br)cc1.OB(O)c1cccc2c1oc1ccccc12>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.C1(=CC=CC=C1)C.C(C)O>C[Si](C)(C)c1ccc(-c2cccc3c2oc2ccccc23)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c4a20bd2579a469cb008df46655d2422
CC(C)(C)OC(=O)NC(Cc1ccc(I)cc1)C(=O)O.CI>>COC(=O)C(Cc1ccc(I)cc1)NC(=O)OC(C)(C)C
IC.C(C)(C)(C)OC(=O)NC(C(=O)O)CC1=CC=C(C=C1)I.C(=O)([O-])[O-].[K+].[K+]>>COC(C(CC1=CC=C(C=C1)I)NC(=O)OC(C)(C)C)=O
[OH:2][C:3](=[O:4])[CH:5]([CH2:6][c:7]1[cH:8][cH:9][c:10]([I:11])[cH:12][cH:13]1)[NH:14][C:15](=[O:16])[O:17][C:18]([CH3:19])([CH3:20])[CH3:21].I[CH3:1]>>[CH3:1][O:2][C:3](=[O:4])[CH:5]([CH2:6][c:7]1[cH:8][cH:9][c:10]([I:11])[cH:12][cH:13]1)[NH:14][C:15](=[O:16])[O:17][C:18]([CH3:19])([CH3:20])[CH3:21]
CC(C)(C)OC(=O)NC(Cc1ccc(I)cc1)C(=O)O.CI
COC(=O)C(Cc1ccc(I)cc1)NC(=O)OC(C)(C)C
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
9474aa79a2adc7353c0c02444ca598a6f486ecdd7ed5edb9ae0645721ee50389
badd4f82161bb0ee7acffd023ea4caae5d036bce7065c10ab0a06e83a6a6f119
c1ccccc1
I-[CH3;D1;+0:1].[C:2]-[C:3](=[O;D1;H0:4])-[OH;D1;+0:5]>>[C:2]-[C:3](=[O;D1;H0:4])-[O;H0;D2;+0:5]-[CH3;D1;+0:1]
110.7
[{"value": 98.0, "product": "COC(C(CC1=CC=C(C=C1)I)NC(=O)OC(C)(C)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 110.7, "product": "COC(C(CC1=CC=C(C=C1)I)NC(=O)OC(C)(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
15
MINUTE
A solution of 2-tert-butoxycarbonylamino-3-(4-iodophenyl)-propanoic acid (5.0 g, 12.8 mmol) in DMF (50 mL) was treated with K2CO3 (2.2 g, 15.4 mmol). After stirring for 15 min, the solution was cooled to 0° C. and treated with iodomethane (1.0 mL, 15.4 mmol) After the addition was complete, the reaction mixture was sti...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Ester
null
null
c1ccccc1
HI
CN(C)C=O
0
0.25
CC(C)(C)OC(=O)NC(Cc1ccc(I)cc1)C(=O)O.CI>CN(C)C=O>COC(=O)C(Cc1ccc(I)cc1)NC(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c1e6650e50484852b3b264bedba24929
COC(=O)C(Cc1ccc(I)cc1)NC(=O)OC(C)(C)C.OB(O)c1ccc(-c2cccc3c2oc2ccccc23)cc1>>COC(=O)C(Cc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)OC(C)(C)C
COC(C(CC1=CC=C(C=C1)I)NC(=O)OC(C)(C)C)=O.C1=CC=C(C=2OC3=C(C21)C=CC=C3)C3=CC=C(C=C3)B(O)O.C(=O)([O-])[O-].[K+].[K+]>>COC(C(CC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1)NC(=O)OC(C)(C)C)=O
I[c:10]1[cH:9][cH:8][c:7]([CH2:6][CH:5]([C:3]([O:2][CH3:1])=[O:4])[NH:32][C:33](=[O:34])[O:35][C:36]([CH3:37])([CH3:38])[CH3:39])[cH:31][cH:30]1.OB(O)[c:11]1[cH:12][cH:13][c:14](-[c:15]2[cH:16][cH:17][cH:18][c:19]3[c:20]2[o:21][c:22]2[cH:23][cH:24][cH:25][cH:26][c:27]32)[cH:28][cH:29]1>>[CH3:1][O:2][C:3](=[O:4])[CH:5](...
COC(=O)C(Cc1ccc(I)cc1)NC(=O)OC(C)(C)C.OB(O)c1ccc(-c2cccc3c2oc2ccccc23)cc1
COC(=O)C(Cc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)OC(C)(C)C
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
C1(=CC=CC=C1)C.C(C)(=O)OCC.C(C)O
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
I-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:8]:[c:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9]:[c:10]
70.3
[{"value": 70.0, "product": "COC(C(CC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1)NC(=O)OC(C)(C)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 70.3, "product": "COC(C(CC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1)NC(=O)OC(C)(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": fal...
null
null
null
null
A solution of 2-tert-Butoxycarbonylamino-3-(4-iodophenyl)-propanoic acid methyl ester (1.22 g, 3 mmol), 4-(4-dibenzofuranyl)benzeneboronic acid (0.906 g, 3.15 mmol) and Pd(PPh3)4 (160 mg, 5 mol %) in toluene (25 mL) and ethanol (6.0 mL) was treated with 2 M K2CO3 (4.5 mL). The reaction mixture was heated to reflux for ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1.c1ccc2c(c1)oc1ccccc12
HI.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C1(=CC=CC=C1)C.C(C)(=O)OCC.C(C)O
null
null
COC(=O)C(Cc1ccc(I)cc1)NC(=O)OC(C)(C)C.OB(O)c1ccc(-c2cccc3c2oc2ccccc23)cc1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C1(=CC=CC=C1)C.C(C)(=O)OCC.C(C)O>COC(=O)C(Cc1ccc(-c2ccc(-c3cccc4c3oc3ccccc3...
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d1f2ad0e7d754a7eb8022375fb43e47c
COC(=O)C(Cc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)OC(C)(C)C>>CC(C)(C)OC(=O)NC(Cc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
COC(C(CC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1)NC(=O)OC(C)(C)C)=O.[OH-].[K+].Cl>>C(C)(C)(C)OC(=O)NC(C(=O)O)CC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1
C[O:38][C:36]([CH:9]([NH:8][C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[CH2:10][c:11]1[cH:12][cH:13][c:14](-[c:15]2[cH:16][cH:17][c:18](-[c:19]3[cH:20][cH:21][cH:22][c:23]4[c:24]3[o:25][c:26]3[cH:27][cH:28][cH:29][cH:30][c:31]43)[cH:32][cH:33]2)[cH:34][cH:35]1)=[O:37]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:...
COC(=O)C(Cc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)OC(C)(C)C
CC(C)(C)OC(=O)NC(Cc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
null
null
CO.C(C)(=O)OCC.C1CCOC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
67
[{"value": 67.0, "product": "C(C)(C)(C)OC(=O)NC(C(=O)O)CC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 65.7, "product": "C(C)(C)(C)OC(=O)NC(C(=O)O)CC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": f...
null
null
1
HOUR
A solution of 2-tert-butoxycarbonylamino-3-(4′-dibenzofuran-4-yl-biphen-4-yl)-propanoic acid methyl ester (125 mg, 0.24 mmol) in THF (2 mL) and methanol (2 mL) was cooled to 0° C. and treated with 2 N KOH (1.0 mL). After stirring at room temperature for 1 h the solution was acidified with 10% HCl to pH 2 and diluted wi...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)oc1ccccc12
Other
CO.C(C)(=O)OCC.C1CCOC1
null
1
COC(=O)C(Cc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)OC(C)(C)C>CO.C(C)(=O)OCC.C1CCOC1>CC(C)(C)OC(=O)NC(Cc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4746e29d97774ab99b4403d390d1b542
CC(C)(C)OC(=O)N[C@@H](CO)C(=O)O.CS(=O)(=O)Cl>>COC(=O)C(CS(C)(=O)=O)NC(=O)OC(C)(C)C
Cl.C(C)(C)(C)OC(=O)N[C@@H](CO)C(=O)O.C(C)N(CC)CC.CS(=O)(=O)Cl>>COC(C(CS(=O)(=O)C)NC(=O)OC(C)(C)C)=O
O[CH2:6][C@@H:5]([C:3]([OH:2])=[O:4])[NH:11][C:12](=[O:13])[O:14][C:15]([CH3:16])([CH3:17])[CH3:18].Cl[S:7]([CH3:8])(=[O:9])=[O:10]>>[CH3:1][O:2][C:3](=[O:4])[CH:5]([CH2:6][S:7]([CH3:8])(=[O:9])=[O:10])[NH:11][C:12](=[O:13])[O:14][C:15]([CH3:16])([CH3:17])[CH3:18]
CC(C)(C)OC(=O)N[C@@H](CO)C(=O)O.CS(=O)(=O)Cl
COC(=O)C(CS(C)(=O)=O)NC(=O)OC(C)(C)C
null
null
ClCCl
Acylation
OtherReaction
f340fda5ddb0801f9d294237f8b5aa464e0f39c22881cfcbf8ee50f8e31debc0
59e7803dc5747eb096367d38cb340b4bd5044ddb99993781a2b4a889032ab5b2
null
Cl-[S;H0;D4;+0:1](-[C;D1;H3:2])(=[O;D1;H0:3])=[O;D1;H0:4].O-[CH2;D2;+0:5]-[C@H;D3;+0:6](-[#7:7]-[C:8](=[O;D1;H0:9])-[#8:10]-[C:11](-[C;D1;H3:12])(-[C;D1;H3:13])-[C;D1;H3:14])-[C:15](=[O;D1;H0:16])-[OH;D1;+0:17]>>[C;D1;H3:12]-[C:11](-[C;D1;H3:13])(-[C;D1;H3:14])-[#8:10]-[C:8](=[O;D1;H0:9])-[#7:7]-[CH;D3;+0:6](-[CH2;D2;+...
88.9
[{"value": 84.0, "product": "COC(C(CS(=O)(=O)C)NC(=O)OC(C)(C)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 88.9, "product": "COC(C(CS(=O)(=O)C)NC(=O)OC(C)(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
A solution of N-tert-butoxycarbonylserine (1.1 g, 5.0 mmol) and triethylamine (0.84 mL, 6.0 mmol) in dichloromethane (50 mL) was cooled to 0° C. and treated with methylsulfonyl chloride (0.44 mL, 5.8 mmol)). After stirring an additional 2 h, the reaction mixture was acidified with 2% HCl (20 mL) and extracted with dich...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary alcohol.Sulfonyl halide
Ester.Sulfone
null
null
null
Other
ClCCl
null
2
CC(C)(C)OC(=O)N[C@@H](CO)C(=O)O.CS(=O)(=O)Cl>ClCCl>COC(=O)C(CS(C)(=O)=O)NC(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f470bd2d0d19441fb55111aeb427b95d
COC(=O)C(CS(C)(=O)=O)NC(=O)OC(C)(C)C.Sc1ccc(Br)cc1>>COC(=O)C(CSc1ccc(Br)cc1)NC(=O)OC(C)(C)C
Cl.COC(C(CS(=O)(=O)C)NC(=O)OC(C)(C)C)=O.BrC1=CC=C(C=C1)S.C(=O)([O-])[O-].[Cs+].[Cs+]>>COC(C(CSC1=CC=C(C=C1)Br)NC(=O)OC(C)(C)C)=O
CS(=O)(=O)[CH2:6][CH:5]([C:3]([O:2][CH3:1])=[O:4])[NH:15][C:16](=[O:17])[O:18][C:19]([CH3:20])([CH3:21])[CH3:22].[SH:7][c:8]1[cH:9][cH:10][c:11]([Br:12])[cH:13][cH:14]1>>[CH3:1][O:2][C:3](=[O:4])[CH:5]([CH2:6][S:7][c:8]1[cH:9][cH:10][c:11]([Br:12])[cH:13][cH:14]1)[NH:15][C:16](=[O:17])[O:18][C:19]([CH3:20])([CH3:21])[C...
COC(=O)C(CS(C)(=O)=O)NC(=O)OC(C)(C)C.Sc1ccc(Br)cc1
COC(=O)C(CSc1ccc(Br)cc1)NC(=O)OC(C)(C)C
null
null
CN(C)C=O.C(C)(=O)OCC
Heteroatom Alkylation and Arylation
OtherReaction
4192b8e9846f9aa599819ba0483e36bc07a5d02e0fa0c81cf986e2b744c178e4
f2e0bb31edbeb92a7317d787d4b892418ccdf9fe3a4c00c7fbe8e3075b7e8833
c1ccccc1
C-S(=O)(=O)-[CH2;D2;+0:1]-[C:2](-[#7:3]-[C:4](=[O;D1;H0:5])-[#8:6]-[C:7](-[C;D1;H3:8])(-[C;D1;H3:9])-[C;D1;H3:10])-[C:11](=[O;D1;H0:12])-[#8:13]-[C;D1;H3:14].[SH;D1;+0:15]-[c:16](:[c:17]):[c:18]>>[C;D1;H3:14]-[#8:13]-[C:11](=[O;D1;H0:12])-[C:2](-[#7:3]-[C:4](=[O;D1;H0:5])-[#8:6]-[C:7](-[C;D1;H3:8])(-[C;D1;H3:9])-[C;D1;...
76
[{"value": 76.0, "product": "COC(C(CSC1=CC=C(C=C1)Br)NC(=O)OC(C)(C)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 76.0, "product": "COC(C(CSC1=CC=C(C=C1)Br)NC(=O)OC(C)(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
Solution of 2-tert-Butoxycarbonylamino-3-methylsulfonylpropanoic acid methyl ester (0.86 g, 2.89 mmol) and 4-bromobenzenthiol (0.56 g, 2.89 mmol) in DMF (10 mL) was cooled to at 0° C. and treated with Cs2CO3 (1.1 g, 3.2 mmol). After stirring at room temperature for 2 h, the reaction was acidified with 5% HCl (15 mL) an...
10.6084/m9.figshare.5104873.v1
null
Aromatic thiol.Sulfone
Monosulfide
null
null
c1ccccc1
HO-
CN(C)C=O.C(C)(=O)OCC
null
2
COC(=O)C(CS(C)(=O)=O)NC(=O)OC(C)(C)C.Sc1ccc(Br)cc1>CN(C)C=O.C(C)(=O)OCC>COC(=O)C(CSc1ccc(Br)cc1)NC(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ea35a83fce73409183c02a33f4f806f0
COC(=O)C(CSc1ccc(Br)cc1)NC(=O)OC(C)(C)C.OB(O)c1ccc(-c2cccc3c2oc2ccccc23)cc1>>COC(=O)C(CSc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)OC(C)(C)C
COC(C(CSC1=CC=C(C=C1)Br)NC(=O)OC(C)(C)C)=O.C1=CC=C(C=2OC3=C(C21)C=CC=C3)C3=CC=C(C=C3)B(O)O.C(=O)([O-])[O-].[K+].[K+]>>COC(C(CSC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1)NC(=O)OC(C)(C)C)=O
Br[c:11]1[cH:10][cH:9][c:8]([S:7][CH2:6][CH:5]([C:3]([O:2][CH3:1])=[O:4])[NH:33][C:34](=[O:35])[O:36][C:37]([CH3:38])([CH3:39])[CH3:40])[cH:32][cH:31]1.OB(O)[c:12]1[cH:13][cH:14][c:15](-[c:16]2[cH:17][cH:18][cH:19][c:20]3[c:21]2[o:22][c:23]2[cH:24][cH:25][cH:26][cH:27][c:28]32)[cH:29][cH:30]1>>[CH3:1][O:2][C:3](=[O:4])...
COC(=O)C(CSc1ccc(Br)cc1)NC(=O)OC(C)(C)C.OB(O)c1ccc(-c2cccc3c2oc2ccccc23)cc1
COC(=O)C(CSc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)OC(C)(C)C
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
C1(=CC=CC=C1)C.C(C)(=O)OCC.C(C)O
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:8]:[c:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9]:[c:10]
72
[{"value": 72.0, "product": "COC(C(CSC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1)NC(=O)OC(C)(C)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 70.7, "product": "COC(C(CSC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1)NC(=O)OC(C)(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": f...
null
null
null
null
A solution of 2-tert-Butoxycarbonylamino-3-(4-bromophenylsulfanyl)-propanoic acid methyl ester (0.55 g, 1.41 mmol), 4-(4-dibenzofuranyl)benzeneboronic acid (0.44 g, 1.52 mmol) and Pd(PPh3)4 (0.073 g, 5 mol %) in toluene (15 mL) and ethanol (3.0 mL) was treated with 2 M K2CO3 (2.2 mL). The reaction mixture was heated to...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1.c1ccc2c(c1)oc1ccccc12
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C1(=CC=CC=C1)C.C(C)(=O)OCC.C(C)O
null
null
COC(=O)C(CSc1ccc(Br)cc1)NC(=O)OC(C)(C)C.OB(O)c1ccc(-c2cccc3c2oc2ccccc23)cc1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C1(=CC=CC=C1)C.C(C)(=O)OCC.C(C)O>COC(=O)C(CSc1ccc(-c2ccc(-c3cccc4c3oc3ccc...
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-435cf321ee11435b869150c33a1c4555
COC(=O)C(CSc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)OC(C)(C)C>>CC(C)(C)OC(=O)NC(CSc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
COC(C(CSC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1)NC(=O)OC(C)(C)C)=O.[OH-].[K+].Cl>>C(C)(C)(C)OC(=O)NC(C(=O)O)CSC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1
C[O:39][C:37]([CH:9]([NH:8][C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[CH2:10][S:11][c:12]1[cH:13][cH:14][c:15](-[c:16]2[cH:17][cH:18][c:19](-[c:20]3[cH:21][cH:22][cH:23][c:24]4[c:25]3[o:26][c:27]3[cH:28][cH:29][cH:30][cH:31][c:32]43)[cH:33][cH:34]2)[cH:35][cH:36]1)=[O:38]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6...
COC(=O)C(CSc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)OC(C)(C)C
CC(C)(C)OC(=O)NC(CSc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
null
null
CO.C(C)(=O)OCC.C1CCOC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
75.5
[{"value": 75.0, "product": "C(C)(C)(C)OC(=O)NC(C(=O)O)CSC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 75.5, "product": "C(C)(C)(C)OC(=O)NC(C(=O)O)CSC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired":...
null
null
1
HOUR
A solution of 2-tert-Butoxycarbonylamino-3-(4′-dibenzofuran-4-yl-biphen-4-ylsulfanyl)-propanoic acid methyl ester (0.150 g, 0.27 mmol) in THF (2 mL) and methanol (2 mL) was cooled to 0° C. and treated with 2 N KOH (1.0 mL). After stirring at room temperature for 1 h the solution was acidified with 10% HCl to pH 2 and d...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)oc1ccccc12
Other
CO.C(C)(=O)OCC.C1CCOC1
null
1
COC(=O)C(CSc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)NC(=O)OC(C)(C)C>CO.C(C)(=O)OCC.C1CCOC1>CC(C)(C)OC(=O)NC(CSc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1)C(=O)O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d9aa82c76c054259a0a3ebc54c17fbf5
COC(=O)C(NC(=O)OC(C)(C)C)C(C)(C)SCc1ccc(Br)cc1.Cc1ccccc1.OB(O)c1ccc(-c2cccc3c2oc2ccccc23)cc1>>CCCCOC(=O)NC(C(=O)OC)C(C)(C)SCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
COC(C(C(C)(C)SCC1=CC=C(C=C1)Br)NC(=O)OC(C)(C)C)=O.C1=CC=C(C=2OC3=C(C21)C=CC=C3)C3=CC=C(C=C3)B(O)O.C(=O)([O-])[O-].[K+].[K+].C1(=CC=CC=C1)C>>COC(C(C(C)(C)SCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1)NC(=O)OCCCC)=O
C[C:4](C)([CH3:3])[O:5][C:6](=[O:7])[NH:8][CH:9]([C:10](=[O:11])[O:12][CH3:13])[C:14]([CH3:15])([CH3:16])[S:17][CH2:18][c:19]1[cH:20][cH:21][c:22](Br)[cH:42][cH:43]1.Cc1ccc[cH:2][cH:1]1.OB(O)[c:23]1[cH:24][cH:25][c:26](-[c:27]2[cH:28][cH:29][cH:30][c:31]3[c:32]2[o:33][c:34]2[cH:35][cH:36][cH:37][cH:38][c:39]32)[cH:40][...
COC(=O)C(NC(=O)OC(C)(C)C)C(C)(C)SCc1ccc(Br)cc1.Cc1ccccc1.OB(O)c1ccc(-c2cccc3c2oc2ccccc23)cc1
CCCCOC(=O)NC(C(=O)OC)C(C)(C)SCc1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
C(C)(=O)OCC.C(C)O
C-C Coupling
OtherReaction
5e550543c7c565dfa80df90145ddb8fa53a35e733978f9e0c5f360f8b3b8f5e3
9fc696656adfb7f4ae6a873f93ff0ac2e287a4da8334f055d43ea90269917e79
c1ccc(-c2ccc(-c3cccc4c3oc3ccccc34)cc2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].C-[C;H0;D4;+0:6](-C)(-[CH3;D1;+0:7])-[#8:8]-[C:9](-[#7:10])=[O;D1;H0:11].C-c1:[cH;D2;+0:12]:[cH;D2;+0:13]:c:c:c:1.O-B(-O)-[c;H0;D3;+0:14](:[c:15]:[c:16]):[c:17]:[c:18]>>[#7:10]-[C:9](=[O;D1;H0:11])-[#8:8]-[CH2;D2;+0:6]-[CH2;D2;+0:7]-[CH2;D2;+0:13]-[CH3;D1;+0:12].[c:3]:[c:2]:[...
72
[{"value": 72.0, "product": "COC(C(C(C)(C)SCC1=CC=C(C=C1)C1=CC=C(C=C1)C1=CC=CC2=C1OC1=C2C=CC=C1)NC(=O)OCCCC)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 2-tert-butoxycarbonylamino-3-(4-bromophenylmethylsulfanyl)-3,3-dimethylpropanoic acid methyl ester (0.432 g, 1 mmol), 4-(4-dibenzofuranyl)benzeneboronic acid (0.305 g, 1.05 mmol) and Pd(PPh3)4 (0.052 g, 5 mol %) in toluene (10 mL) and ethanol (3.0 mL) was treated with 2 M K2CO3 (1.5 mL). The reaction mixt...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ether.Boronic acid.Boc
Ether
c1ccccc1.c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1.c1ccc2c(c1)oc1ccccc12
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C(C)(=O)OCC.C(C)O
null
null
COC(=O)C(NC(=O)OC(C)(C)C)C(C)(C)SCc1ccc(Br)cc1.Cc1ccccc1.OB(O)c1ccc(-c2cccc3c2oc2ccccc23)cc1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C(C)(=O)OCC.C(C)O>CCCCOC(=O)NC(C(=O)OC)C(C)(C)SCc1ccc(-c...
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2cedbaf4b2594034ab946f7c953de0a0
Brc1cccc(I)c1.OB(O)c1cccc2c1oc1ccccc12>>Brc1cccc(-c2cccc3c2oc2ccccc23)c1
C1=CC=C(C=2OC3=C(C21)C=CC=C3)B(O)O.BrC1=CC(=CC=C1)I.C(=O)([O-])[O-].[Na+].[Na+]>>BrC=1C=C(C=CC1)C1=CC=CC2=C1OC1=C2C=CC=C1
I[c:6]1[cH:5][cH:4][cH:3][c:2]([Br:1])[cH:20]1.OB(O)[c:7]1[cH:8][cH:9][cH:10][c:11]2[c:12]1[o:13][c:14]1[cH:15][cH:16][cH:17][cH:18][c:19]21>>[Br:1][c:2]1[cH:3][cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][c:11]3[c:12]2[o:13][c:14]2[cH:15][cH:16][cH:17][cH:18][c:19]32)[cH:20]1
Brc1cccc(I)c1.OB(O)c1cccc2c1oc1ccccc12
Brc1cccc(-c2cccc3c2oc2ccccc23)c1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.C1(=CC=CC=C1)C.C(C)(=O)OCC.C(C)O
C-C Coupling
Suzuki coupling with boronic acids
a34fd3f8e97b635d120df300575865eab1505627afd99c75ec2034d5929796bd
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2cccc3c2oc2ccccc23)cc1
I-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9](:[c:10]):[#8;a:11]:[c:12]>>[c:10]:[c:9](:[#8;a:11]:[c:12]):[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:7]:[c:8]
null
[]
80
CELSIUS
null
null
A mixture of 4-dibenzofuranboronic acid (51 mmol), 1-Bromo-3-iodo-benzene (51 mmol), and Pd(PPh3)4, (4 mmol) in 250 mL of toluene and 150 mL of ethanol was heated to obtain a clear solution, then Na2CO3 (155 mmol) in 250 mL water was added. The reaction mixture refluxed for 4 h at 80° C. The mixture was cooled to room ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccc2c(c1)oc1ccccc12
c1ccccc1.c1ccc2c(c1)oc1ccccc12
c1ccccc1.c1ccc2c(c1)oc1ccccc12
HI.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.C1(=CC=CC=C1)C.C(C)(=O)OCC.C(C)O
80
null
Brc1cccc(I)c1.OB(O)c1cccc2c1oc1ccccc12>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.C1(=CC=CC=C1)C.C(C)(=O)OCC.C(C)O>Brc1cccc(-c2cccc3c2oc2ccccc23)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-601a9a85a17547e6be9054fa64ff6c66
Brc1cccc(-c2cccc3c2oc2ccccc23)c1.OB(O)c1ccc(O)cc1>>Oc1ccc(-c2cccc(-c3cccc4c3oc3ccccc34)c2)cc1
Cl.C(=O)([O-])[O-].[Na+].[Na+].BrC=1C=C(C=CC1)C1=CC=CC2=C1OC1=C2C=CC=C1.OC1=CC=C(C=C1)B(O)O>>C1=CC=C(C=2OC3=C(C21)C=CC=C3)C=3C=C(C=CC3)C3=CC=C(C=C3)O
Br[c:6]1[cH:7][cH:8][cH:9][c:10](-[c:11]2[cH:12][cH:13][cH:14][c:15]3[c:16]2[o:17][c:18]2[cH:19][cH:20][cH:21][cH:22][c:23]32)[cH:24]1.OB(O)[c:5]1[cH:4][cH:3][c:2]([OH:1])[cH:26][cH:25]1>>[OH:1][c:2]1[cH:3][cH:4][c:5](-[c:6]2[cH:7][cH:8][cH:9][c:10](-[c:11]3[cH:12][cH:13][cH:14][c:15]4[c:16]3[o:17][c:18]3[cH:19][cH:20]...
Brc1cccc(-c2cccc3c2oc2ccccc23)c1.OB(O)c1ccc(O)cc1
Oc1ccc(-c2cccc(-c3cccc4c3oc3ccccc34)c2)cc1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.C1(=CC=CC=C1)C.C(C)(=O)OCC.C(C)O
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2cccc(-c3cccc4c3oc3ccccc34)c2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:4]:[c:5]
null
[]
80
CELSIUS
null
null
A mixture of 4-(3-bromo-phenyl)-dibenzofuran (0.62 mmol), 4-hydroxyphenyl boronic acid (0.62 mmol), and Pd(PPh3)4, (0.05 mmol) in 2 mL of toluene and 1 mL ethanol was heated to obtain a clear solution, then Na2CO3 (1.9 mmol) in 2 mL water was added. The reaction mixture refluxed for 5 h at 80° C. The mixture was cooled...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1.c1ccc2c(c1)oc1ccccc12
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.C1(=CC=CC=C1)C.C(C)(=O)OCC.C(C)O
80
null
Brc1cccc(-c2cccc3c2oc2ccccc23)c1.OB(O)c1ccc(O)cc1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.C1(=CC=CC=C1)C.C(C)(=O)OCC.C(C)O>Oc1ccc(-c2cccc(-c3cccc4c3oc3ccccc34)c2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b2cd2207d0084987a974d1c5932b137e
BrCc1cccc(Br)c1.FC(F)(F)c1ccc2c(c1)NCCC2>>FC(F)(F)c1ccc2c(c1)N(Cc1cccc(Br)c1)CCC2
BrC1=CC(=CC=C1)CBr.FC(C1=CC=C2CCCNC2=C1)(F)F.C(C)(=O)[O-].[Na+]>>BrC=1C=C(CN2CCCC3=CC=C(C=C23)C(F)(F)F)C=CC1
Br[CH2:12][c:13]1[cH:14][cH:15][cH:16][c:17]([Br:18])[cH:19]1.[F:1][C:2]([F:3])([F:4])[c:5]1[cH:6][cH:7][c:8]2[c:9]([cH:10]1)[NH:11][CH2:20][CH2:21][CH2:22]2>>[F:1][C:2]([F:3])([F:4])[c:5]1[cH:6][cH:7][c:8]2[c:9]([cH:10]1)[N:11]([CH2:12][c:13]1[cH:14][cH:15][cH:16][c:17]([Br:18])[cH:19]1)[CH2:20][CH2:21][CH2:22]2
BrCc1cccc(Br)c1.FC(F)(F)c1ccc2c(c1)NCCC2
FC(F)(F)c1ccc2c(c1)N(Cc1cccc(Br)c1)CCC2
null
null
O.C(C)O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
219d202b93cb5a235df7e6646f3b9409e60d3c325f1ec37d9b75eb0c3554d20f
523d37155b42c8dc851abeddadebb241cdd90bdf649ba750c35e13c8c752d7b0
c1ccc(CN2CCCc3ccccc32)cc1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[C:5]-[C:6]-[NH;D2;+0:7]-[c:8](:[c:9]):[c:10]>>[C:5]-[C:6]-[N;H0;D3;+0:7](-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4])-[c:8](:[c:9]):[c:10]
82
[{"value": 82.0, "product": "BrC=1C=C(CN2CCCC3=CC=C(C=C23)C(F)(F)F)C=CC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 81.9, "product": "BrC=1C=C(CN2CCCC3=CC=C(C=C23)C(F)(F)F)C=CC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
2
HOUR
Under a nitrogen atmosphere, a solution of bromo-3-bromomethyl-benzene (3.47 g, 13.p mmol) and 7-trifluoromethyl-1,2,3,4-tetrahydro-quinoline (2.93 g, 14.6 mmol) in ethanol (15 mL, 1 M) was treated with sodium acetate (5.69 g, 69.3 mmol) and heated to 80° C. After stirring 2 h, the solution was cooled to room temperatu...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amine
Tertiary amine
c1ccc2c(c1)CCCN2
c1ccc2c(c1)CCC[NH]2
c1ccccc1.c1ccc2c(c1)CCC[NH]2
HBr
O.C(C)O
80
2
BrCc1cccc(Br)c1.FC(F)(F)c1ccc2c(c1)NCCC2>O.C(C)O>FC(F)(F)c1ccc2c(c1)N(Cc1cccc(Br)c1)CCC2
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a49809f6e49547d4830ecc1868c240e0
FC(F)(F)c1ccc2c(c1)N(Cc1cccc(Br)c1)CCC2.OCc1ccc(B(O)O)cc1>>OCc1ccc(-c2cccc(CN3CCCc4ccc(C(F)(F)F)cc43)c2)cc1
BrC=1C=C(CN2CCCC3=CC=C(C=C23)C(F)(F)F)C=CC1.OCC1=CC=C(C=C1)B(O)O.C(=O)([O-])[O-].[Na+].[Na+]>>FC(C1=CC=C2CCCN(C2=C1)CC=1C=C(C=CC1)C1=CC=C(C=C1)CO)(F)F
Br[c:7]1[cH:8][cH:9][cH:10][c:11]([CH2:12][N:13]2[CH2:14][CH2:15][CH2:16][c:17]3[cH:18][cH:19][c:20]([C:21]([F:22])([F:23])[F:24])[cH:25][c:26]32)[cH:27]1.OB(O)[c:6]1[cH:5][cH:4][c:3]([CH2:2][OH:1])[cH:29][cH:28]1>>[OH:1][CH2:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][c:11]([CH2:12][N:13]3[CH2:14][CH2:15][CH2...
FC(F)(F)c1ccc2c(c1)N(Cc1cccc(Br)c1)CCC2.OCc1ccc(B(O)O)cc1
OCc1ccc(-c2cccc(CN3CCCc4ccc(C(F)(F)F)cc43)c2)cc1
null
null
C1(=CC=CC=C1)C.C(C)O
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2cccc(CN3CCCc4ccccc43)c2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:4]:[c:5]
null
[]
80
CELSIUS
null
null
Under a nitrogen atmosphere, a solution of 1-(3-bromo-benzyl)-7-trifluoromethyl-1,2,3,4-tetrahydro-quinoline (2.36 g, 6.37 mmol), 4-(hydroxymethyl)phenyl boronic acid (1.07 g, 7.01 mmol), and 2 M Na2CO3 (7 mL, 12.7 mmol) in 16 mL of toluene and 4 mL ethanol (0.3 M) was treated with tetrakistriphenylphosphine palladium ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HBr.B
C1(=CC=CC=C1)C.C(C)O
80
null
FC(F)(F)c1ccc2c(c1)N(Cc1cccc(Br)c1)CCC2.OCc1ccc(B(O)O)cc1>C1(=CC=CC=C1)C.C(C)O>OCc1ccc(-c2cccc(CN3CCCc4ccc(C(F)(F)F)cc43)c2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-167f9e071d6e41f2b5c42031809a40b8
COC(=O)C(CS)NC(=O)OC(C)(C)C.OCc1ccc(-c2cccc(CN3CCCc4ccc(C(F)(F)F)cc43)c2)cc1>>COC(=O)C(CSCc1ccc(-c2cccc(CN3CCCc4ccc(C(F)(F)F)cc43)c2)cc1)NC(=O)OC(C)(C)C
FC(C1=CC=C2CCCN(C2=C1)CC=1C=C(C=CC1)C1=CC=C(C=C1)CO)(F)F.COC(C(CS)NC(=O)OC(C)(C)C)=O.N(=NC(=O)N1CCCCC1)C(=O)N1CCCCC1.N1C=NC=C1.CP(C)C>>COC(C(CSCC1=CC=C(C=C1)C1=CC(=CC=C1)CN1CCCC2=CC=C(C=C12)C(F)(F)F)NC(=O)OC(C)(C)C)=O
[CH3:1][O:2][C:3](=[O:4])[CH:5]([CH2:6][SH:7])[NH:36][C:37](=[O:38])[O:39][C:40]([CH3:41])([CH3:42])[CH3:43].O[CH2:8][c:9]1[cH:10][cH:11][c:12](-[c:13]2[cH:14][cH:15][cH:16][c:17]([CH2:18][N:19]3[CH2:20][CH2:21][CH2:22][c:23]4[cH:24][cH:25][c:26]([C:27]([F:28])([F:29])[F:30])[cH:31][c:32]43)[cH:33]2)[cH:34][cH:35]1>>[C...
COC(=O)C(CS)NC(=O)OC(C)(C)C.OCc1ccc(-c2cccc(CN3CCCc4ccc(C(F)(F)F)cc43)c2)cc1
COC(=O)C(CSCc1ccc(-c2cccc(CN3CCCc4ccc(C(F)(F)F)cc43)c2)cc1)NC(=O)OC(C)(C)C
null
null
ClCCl.CCCCCCC
Heteroatom Alkylation and Arylation
OtherReaction
94a14d3014f7fdb5c4fa6f9f37d523bd85860ea21497647c55ba9393bbc36835
f8355ba7e68f7d5b10019904f32df628ca7b7bc14adae6579e7d0de9afb40579
c1ccc(-c2cccc(CN3CCCc4ccccc43)c2)cc1
O-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[#8:5]-[C:6](=[O;D1;H0:7])-[C:8]-[C:9]-[SH;D1;+0:10]>>[#8:5]-[C:6](=[O;D1;H0:7])-[C:8]-[C:9]-[S;H0;D2;+0:10]-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
1
HOUR
Under a nitrogen atmosphere, a solution of [3′-(7-trifluoromethyl-3,4-dihydro-2H-quinolin-1-ylmethyl)-biphenyl-4-yl]-methanol (0.257 g, 0.65 mmol), 2-tert-butoxycarbonylamino-3-mercapto-propionic acid methyl ester (0.304 g, 1.29 mmol), 1,1′-(azodicarbonyl)dipiperidine (0.343 g, 1.36 mmol), and imidazole (0.92 g, 1.36 m...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Aliphatic thiol
Monosulfide
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HO-
ClCCl.CCCCCCC
null
1
COC(=O)C(CS)NC(=O)OC(C)(C)C.OCc1ccc(-c2cccc(CN3CCCc4ccc(C(F)(F)F)cc43)c2)cc1>ClCCl.CCCCCCC>COC(=O)C(CSCc1ccc(-c2cccc(CN3CCCc4ccc(C(F)(F)F)cc43)c2)cc1)NC(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2a561daa93bc41678b94a936453b3b2f
COC(=O)C(CSCc1ccc(-c2cccc(CN3CCCc4ccc(C(F)(F)F)cc43)c2)cc1)NC(=O)OC(C)(C)C>>CC(C)(C)OC(=O)NC(CSCc1ccc(-c2cccc(CN3CCCc4ccc(C(F)(F)F)cc43)c2)cc1)C(=O)O
COC(C(CSCC1=CC=C(C=C1)C1=CC(=CC=C1)CN1CCCC2=CC=C(C=C12)C(F)(F)F)NC(=O)OC(C)(C)C)=O.[OH-].[Na+].Cl>>C(C)(C)(C)OC(=O)NC(C(=O)O)CSCC1=CC=C(C=C1)C1=CC(=CC=C1)CN1CCCC2=CC=C(C=C12)C(F)(F)F
C[O:42][C:40]([CH:9]([NH:8][C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[CH2:10][S:11][CH2:12][c:13]1[cH:14][cH:15][c:16](-[c:17]2[cH:18][cH:19][cH:20][c:21]([CH2:22][N:23]3[CH2:24][CH2:25][CH2:26][c:27]4[cH:28][cH:29][c:30]([C:31]([F:32])([F:33])[F:34])[cH:35][c:36]43)[cH:37]2)[cH:38][cH:39]1)=[O:41]>>[CH3:1][C:2]...
COC(=O)C(CSCc1ccc(-c2cccc(CN3CCCc4ccc(C(F)(F)F)cc43)c2)cc1)NC(=O)OC(C)(C)C
CC(C)(C)OC(=O)NC(CSCc1ccc(-c2cccc(CN3CCCc4ccc(C(F)(F)F)cc43)c2)cc1)C(=O)O
null
null
CO.C1CCOC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(-c2cccc(CN3CCCc4ccccc43)c2)cc1
C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
null
[]
null
null
3
HOUR
Under a nitrogen atmosphere, a solution of 2-tert-butoxycarbonylamino-3-[3′-(7-trifluoromethyl-3,4-dihydro-2H-quinolin-1-ylmethyl)-biphenyl-4-ylmethylsulfanyl]-propionic acid methyl ester (0.173 g, 0.281 mmol) in 4 mL of THF and 1 mL of methanol was treated with 2 N NaOH (1.5 mL, 2.81 mmol). After stirring at room temp...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
Other
CO.C1CCOC1
null
3
COC(=O)C(CSCc1ccc(-c2cccc(CN3CCCc4ccc(C(F)(F)F)cc43)c2)cc1)NC(=O)OC(C)(C)C>CO.C1CCOC1>CC(C)(C)OC(=O)NC(CSCc1ccc(-c2cccc(CN3CCCc4ccc(C(F)(F)F)cc43)c2)cc1)C(=O)O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-70823f437a944b05a91f156fe600ec4b
CC(C)(C)OC(=O)NN.O=C1CCN(C(=O)OCC2c3ccccc3-c3ccccc32)CC1>>CC(C)(C)OC(=O)NN=C1CCN(C(=O)OCC2c3ccccc3-c3ccccc32)CC1
C1=CC=CC=2C3=CC=CC=C3C(C12)COC(=O)N1CCC(CC1)=O.N(N)C(=O)OC(C)(C)C>>CC(C)(OC(=O)NN=C1CCN(CC1)C(=O)OCC1C2=CC=CC=C2C=2C=CC=CC12)C
[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[NH:8][NH2:9].O=[C:10]1[CH2:11][CH2:12][N:13]([C:14](=[O:15])[O:16][CH2:17][CH:18]2[c:19]3[cH:20][cH:21][cH:22][cH:23][c:24]3-[c:25]3[cH:26][cH:27][cH:28][cH:29][c:30]32)[CH2:31][CH2:32]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[NH:8][N:9]=[C:10]1[CH2:11][CH2:12]...
CC(C)(C)OC(=O)NN.O=C1CCN(C(=O)OCC2c3ccccc3-c3ccccc32)CC1
CC(C)(C)OC(=O)NN=C1CCN(C(=O)OCC2c3ccccc3-c3ccccc32)CC1
null
null
C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
c65f0bc70664fcfce830ed71426d33f4ad8e3395c2675dbe7ef04b365fe00b18
ac24b4d8621c562f7730855d0c8234199dd2eb11db82411f7f92e5c96064c963
N=C1CCN(C(=O)OCC2c3ccccc3-c3ccccc32)CC1
O=[C;H0;D3;+0:1]1-[C:2]-[C:3]-[#7:4]-[C:5]-[C:6]-1.[C;D1;H3:7]-[C:8](-[C;D1;H3:9])(-[C;D1;H3:10])-[#8:11]-[C:12](=[O;D1;H0:13])-[#7:14]-[NH2;D1;+0:15]>>[C;D1;H3:7]-[C:8](-[C;D1;H3:9])(-[C;D1;H3:10])-[#8:11]-[C:12](=[O;D1;H0:13])-[#7:14]-[N;H0;D2;+0:15]=[C;H0;D3;+0:1]1-[C:2]-[C:3]-[#7:4]-[C:5]-[C:6]-1
null
[]
null
null
null
null
A mixture of 16.0 g (0.05 mol) of 1-(9H-fluoren-9-ylmethoxycarbonyl)-4-piperidinone, 7.25 g (0.055 mol) of tert. butyl hydrazinoformate and 250 ml of ethanol was refluxed for 1 hour. The solvent was distilled off in vacuo, the oily residue remaining was triturated with diethylether. The crystalline precipitate thus for...
10.6084/m9.figshare.5104873.v1
null
Acylhydrazine.Ketone
Hydrazone amide
C1CC[NH]CC1
C1CC[NH]CC1
C1CC[NH]CC1.c1ccc2c(c1)Cc1ccccc12
HO-
C(C)O
null
null
CC(C)(C)OC(=O)NN.O=C1CCN(C(=O)OCC2c3ccccc3-c3ccccc32)CC1>C(C)O>CC(C)(C)OC(=O)NN=C1CCN(C(=O)OCC2c3ccccc3-c3ccccc32)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c53bb0e510fb4a73be010faee4a6d4a9
CC(C)(C)OC(=O)NNC1CCN(C(=O)OCC2c3ccccc3-c3ccccc32)CC1>>NNC1CCN(C(=O)OCC2c3ccccc3-c3ccccc32)CC1
CC(C)(OC(=O)NNC1CCN(CC1)C(=O)OCC1C2=CC=CC=C2C=2C=CC=CC12)C.Cl.Cl>>Cl.C1=CC=CC=2C3=CC=CC=C3C(C12)COC(=O)N1CCC(CC1)NN
CC(C)(C)OC(=O)[NH:2][NH:3][CH:4]1[CH2:5][CH2:6][N:7]([C:8](=[O:9])[O:10][CH2:11][CH:12]2[c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]3-[c:19]3[cH:20][cH:21][cH:22][cH:23][c:24]32)[CH2:25][CH2:26]1>>[NH2:2][NH:3][CH:4]1[CH2:5][CH2:6][N:7]([C:8](=[O:9])[O:10][CH2:11][CH:12]2[c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]3-[c:19]3[...
CC(C)(C)OC(=O)NNC1CCN(C(=O)OCC2c3ccccc3-c3ccccc32)CC1
NNC1CCN(C(=O)OCC2c3ccccc3-c3ccccc32)CC1
null
null
FC(C(=O)O)(F)F.C(C)(=O)OCC
Reduction
Reduction of primary amides to amines
39e11744340ea5c8f4187a9034f8b9800b3b6ccbfd7b2876214303dc07bb979f
2249bb4c64fe4943bfcef5de0ada6c23bea6dec24992f87f55d0785b30b30b5a
O=C(OCC1c2ccccc2-c2ccccc21)N1CCCCC1
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[#7:2]-[C:3]>>[C:3]-[#7:2]-[NH2;D1;+0:1]
null
[]
null
null
1
HOUR
21.8 g (0.0498 mol) of N-(1,1-dimethylethoxycarbonyl)-N′-[1-(9H-fluoren-9-ylmethoxycarbonyl)-4-piperidinyl]-hydrazine were dissolved in 100 ml of trifluoroacetic acid and stirred for 1 hour at room temperature. The excess trifluoroacetic acid was removed in vacuo, the residue was dissolved in 50 ml of water and made al...
10.6084/m9.figshare.5104873.v1
null
Acylhydrazine.Carbamic ester.Ether.Boc
Hydrazine
null
null
C1CC[NH]CC1.c1ccc2c(c1)Cc1ccccc12
HO-
FC(C(=O)O)(F)F.C(C)(=O)OCC
null
1
CC(C)(C)OC(=O)NNC1CCN(C(=O)OCC2c3ccccc3-c3ccccc32)CC1>FC(C(=O)O)(F)F.C(C)(=O)OCC>NNC1CCN(C(=O)OCC2c3ccccc3-c3ccccc32)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-fcb9f893e85643fa826eef35bcb0e1ab
C1CCOC1.C1CCOC1.NNC1CCN(C(=O)OCC2c3ccccc3-c3ccccc32)CC1>>O=C(OCC1c2ccccc2-c2ccccc21)N1CCC(n2nc(-c3ccccc3)[nH]c2=O)CC1
O1CCCC1.C1=CC=CC=2C3=CC=CC=C3C(C12)COC(=O)N1CCC(CC1)NN.S.O1CCCC1>>C1(=CC=CC=C1)C=1NC(N(N1)C1CCN(CC1)C(=O)OCC1C2=CC=CC=C2C=2C=CC=CC12)=O
[CH2:25]1[CH2:26][CH2:27][O:33][CH2:32]1.O1[CH2:24][CH2:28][CH2:29][CH2:30]1.[O:1]=[C:2]([O:3][CH2:4][CH:5]1[c:6]2[cH:7][cH:8][cH:9][cH:10][c:11]2-[c:12]2[cH:13][cH:14][cH:15][cH:16][c:17]21)[N:18]1[CH2:19][CH2:20][CH:21]([NH:22][NH2:23])[CH2:34][CH2:35]1>>[O:1]=[C:2]([O:3][CH2:4][CH:5]1[c:6]2[cH:7][cH:8][cH:9][cH:10][...
C1CCOC1.C1CCOC1.NNC1CCN(C(=O)OCC2c3ccccc3-c3ccccc32)CC1
O=C(OCC1c2ccccc2-c2ccccc21)N1CCC(n2nc(-c3ccccc3)[nH]c2=O)CC1
null
null
null
Aromatic Heterocycle Formation
OtherReaction
55694136454ea5ff34e514d0cb673e9c4e0c5e49262f03f99def3591d5f64421
698ca8f9fc42fbe71c5a41554d6cf45f43ec89e80787604700bb38bda168cae4
O=C(OCC1c2ccccc2-c2ccccc21)N1CCC(n2nc(-c3ccccc3)[nH]c2=O)CC1
O1-[CH2;D2;+0:1]-[CH2;D2;+0:2]-[CH2;D2;+0:3]-[CH2;D2;+0:4]-1.[CH2;D2;+0:5]1-[CH2;D2;+0:6]-[CH2;D2;+0:7]-[O;H0;D2;+0:8]-[CH2;D2;+0:9]-1.[C:10]-[C:11](-[NH;D2;+0:12]-[NH2;D1;+0:13])-[C:14]>>[C:10]-[C:11](-[n;H0;D3;+0:12]1:[n;H0;D2;+0:13]:[c;H0;D3;+0:1](-[c;H0;D3;+0:5]2:[cH;D2;+0:6]:[cH;D2;+0:7]:[cH;D2;+0:2]:[cH;D2;+0:3]:...
null
[]
null
null
null
null
The solutions of 5.56 g (0.0165 mol) of [1-(9H-fluoren-9-ylmethoxycarbonyl)-4-piperidinyl]-hydrazine in 60 ml of tetrahydrofuran and 3.7 g (0.0177 mol) of N-(ethoxycarbonyl)-benzothionamide in 30 ml of tetrahydrofuran were combined and refluxed for 1 hour, whereupon hydrogen sulphide was released. The solvent was disti...
10.6084/m9.figshare.5104873.v1
null
Hydrazine.Ether.Ether
null
C1CCOC1.C1CCOC1
c1nc[nH]n1.c1ccccc1
C1CC[NH]CC1.c1nc[nH]n1.c1ccccc1.c1ccc2c(c1)Cc1ccccc12
null
null
null
null
C1CCOC1.C1CCOC1.NNC1CCN(C(=O)OCC2c3ccccc3-c3ccccc32)CC1>>O=C(OCC1c2ccccc2-c2ccccc21)N1CCC(n2nc(-c3ccccc3)[nH]c2=O)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9ead69204b774477a7b81d6b89c7fb2e
O=C(OCC1c2ccccc2-c2ccccc21)N1CCC(n2nc(-c3ccccc3)[nH]c2=O)CC1>>COc1cccc(-c2cn(C3CCNCC3)c(=O)[nH]2)c1
C1(=CC=CC=C1)C=1NC(N(N1)C1CCN(CC1)C(=O)OCC1C2=CC=CC=C2C=2C=CC=CC12)=O.O1CCCC1.C(C)NCC>>COC=1C=C(C=CC1)C=1NC(N(C1)C1CCNCC1)=O
O=C(OCC1c2ccccc2-c2ccccc21)[N:14]1[CH2:13][CH2:12][CH:11]([n:10]2n[c:8](-[c:7]3[cH:6][cH:5][cH:4][cH:3][cH:20]3)[nH:19][c:17]2=[O:18])[CH2:16][CH2:15]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7](-[c:8]2[cH:9][n:10]([CH:11]3[CH2:12][CH2:13][NH:14][CH2:15][CH2:16]3)[c:17](=[O:18])[nH:19]2)[cH:20]1
O=C(OCC1c2ccccc2-c2ccccc21)N1CCC(n2nc(-c3ccccc3)[nH]c2=O)CC1
COc1cccc(-c2cn(C3CCNCC3)c(=O)[nH]2)c1
null
null
CO
Miscellaneous
OtherReaction
3da7a02878e06cc9f6a906874197bfde22e9ae16c883b5c0220ac17f35368816
554d5d10a57a42367e87de6a63897338738b1766c5273ea9d2039a3c5775eef8
O=c1[nH]c(-c2ccccc2)cn1C1CCNCC1
O=C(-O-C-C1-c2:c:c:c:c:c:2-c2:c:c:c:c:c:2-1)-[N;H0;D3;+0:1]1-[C:2]-[C:3]-[C:4](-[n;H0;D3;+0:5]2:n:[c;H0;D3;+0:6](-[c:7]3:[c:8]:[cH;D2;+0:9]:[c:10]:[c:11]:[c:12]:3):[#7;a:13]:[c:14]:2=[O;D1;H0:15])-[C:16]-[C:17]-1>>[C;D1;H3:18]-[#8:19]-[c;H0;D3;+0:9]1:[c:8]:[c:7](-[c;H0;D3;+0:6]2:[#7;a:13]:[c:14](=[O;D1;H0:15]):[n;H0;D3...
null
[]
null
null
30
MINUTE
A mixture of 9.0 g (0.0193 mol) of 2,4-dihydro-5-phenyl-2-[1-(9H-fluoren-9-ylmethoxycarbonyl)-4-piperidinyl]-3H-1,2,4-triazol-3-one, 50 ml of tetrahydrofuran and 70 ml of diethylamine was stirred at room temperature until the end of the reaction monitored by thin layer chromatography. The solvent was removed in vacuo, ...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether
Ether.Secondary amine
C1CC[NH]CC1.c1nc[nH]n1.c1ccccc1.c1ccc2c(c1)Cc1ccccc12
c1ccccc1.c1c[nH]cn1.C1CCNCC1
c1ccccc1.c1c[nH]cn1.C1CCNCC1
HO-
CO
null
0.5
O=C(OCC1c2ccccc2-c2ccccc21)N1CCC(n2nc(-c3ccccc3)[nH]c2=O)CC1>CO>COc1cccc(-c2cn(C3CCNCC3)c(=O)[nH]2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ff6a90c0b5fb4cd7861aa8294d016af9
CC(C)(C)C(=O)Cl.Nc1ccccn1>>CC(C)(C)C(=O)Nc1ccccn1
NC1=NC=CC=C1.C(C)N(CC)CC.C(C(C)(C)C)(=O)Cl>>N1=C(C=CC=C1)NC(C(C)(C)C)=O
Cl[C:5]([C:2]([CH3:1])([CH3:3])[CH3:4])=[O:6].[NH2:7][c:8]1[cH:9][cH:10][cH:11][cH:12][n:13]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[C:5](=[O:6])[NH:7][c:8]1[cH:9][cH:10][cH:11][cH:12][n:13]1
CC(C)(C)C(=O)Cl.Nc1ccccn1
CC(C)(C)C(=O)Nc1ccccn1
null
null
ClCCl
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
c1ccncc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])(-[C;D1;H3:5])-[C;D1;H3:6].[NH2;D1;+0:7]-[c:8](:[c:9]):[#7;a:10]:[c:11]>>[C;D1;H3:4]-[C:3](-[C;D1;H3:5])(-[C;D1;H3:6])-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:7]-[c:8](:[c:9]):[#7;a:10]:[c:11]
null
[]
null
null
2
HOUR
To a solution of 94.1 g (1.0 mol) of 2-aminopyridine and 173 ml (1.25 mol) of triethylamine in 400 ml of dichloromethane were added dropwise, whilst cooling with ice water, 132.5 g (1.099 mol) of pivaloyl chloride in 150 ml of dichloromethane. The. mixture was stirred for 2 hours at room temperature and filtered to rem...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1ccncc1
HCl
ClCCl
null
2
CC(C)(C)C(=O)Cl.Nc1ccccn1>ClCCl>CC(C)(C)C(=O)Nc1ccccn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-34c5e22bc1414db5be821d960eb43398
CN(C)C=O.Nc1ncccc1CNC1CCN(Cc2ccccc2)CC1>>O=C1Nc2ncccc2CN1C1CCN(Cc2ccccc2)CC1
NC1=NC=CC=C1CNC1CCN(CC1)CC1=CC=CC=C1.CN(C=O)C>>C1(=CC=CC=C1)CN1CCC(CC1)N1C(NC2=C(C1)C=CC=N2)=O
CN(C)[CH:2]=[O:1].[NH2:3][c:4]1[n:5][cH:6][cH:7][cH:8][c:9]1[CH2:10][NH:11][CH:12]1[CH2:13][CH2:14][N:15]([CH2:16][c:17]2[cH:18][cH:19][cH:20][cH:21][cH:22]2)[CH2:23][CH2:24]1>>[O:1]=[C:2]1[NH:3][c:4]2[n:5][cH:6][cH:7][cH:8][c:9]2[CH2:10][N:11]1[CH:12]1[CH2:13][CH2:14][N:15]([CH2:16][c:17]2[cH:18][cH:19][cH:20][cH:21][...
CN(C)C=O.Nc1ncccc1CNC1CCN(Cc2ccccc2)CC1
O=C1Nc2ncccc2CN1C1CCN(Cc2ccccc2)CC1
null
null
null
Acylation
OtherReaction
afaddc71d708dfe1a0eeaab802c260059d19c88180ebdb822fd909e0afa6ced6
eebab57e6facb6b0e9da3aa098a8e1cdfa27d9611f85f9a72fe0b16b5e461392
O=C1Nc2ncccc2CN1C1CCN(Cc2ccccc2)CC1
C-N(-C)-[CH;D2;+0:1]=[O;D1;H0:2].[C:3]-[C:4](-[NH;D2;+0:5]-[C:6]-[c:7]:[c:8](-[NH2;D1;+0:9]):[#7;a:10]:[c:11])-[C:12]>>[C:3]-[C:4](-[N;H0;D3;+0:5]1-[C:6]-[c:7]:[c:8](:[#7;a:10]:[c:11])-[NH;D2;+0:9]-[C;H0;D3;+0:1]-1=[O;D1;H0:2])-[C:12]
null
[]
100
CELSIUS
null
null
A mixture of 4.2 g (0.0142 mol) of 2-amino-3-[[[1-(phenylmethyl)-4-piperidinyl]amino]methyl]-pyridine, 2.4 g (0.0148 mol) of N,N′-carbonyldiimidazole and 50 ml of dimethylformamide was heated to 100° C. for 30 minutes. The still warm mixture was stirred into 300 ml of ice water, the precipitate formed was suction filte...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Primary amine.Secondary amine
Urea
null
c1cnc2c(c1)C[NH]CN2
c1cnc2c(c1)C[NH]CN2.C1CC[NH]CC1.c1ccccc1
Other
null
100
null
CN(C)C=O.Nc1ncccc1CNC1CCN(Cc2ccccc2)CC1>>O=C1Nc2ncccc2CN1C1CCN(Cc2ccccc2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-870be06ed5314773b62b576b77a485d7
O=C1Nc2ncccc2CN1C1CCN(Cc2ccccc2)CC1>>O=C1Nc2ncccc2CN1C1CCNCC1
[H][H].C1(=CC=CC=C1)CN1CCC(CC1)N1C(NC2=C(C1)C=CC=N2)=O>>N1CCC(CC1)N1C(NC2=C(C1)C=CC=N2)=O
c1ccc(C[N:15]2[CH2:14][CH2:13][CH:12]([N:11]3[C:2](=[O:1])[NH:3][c:4]4[n:5][cH:6][cH:7][cH:8][c:9]4[CH2:10]3)[CH2:17][CH2:16]2)cc1>>[O:1]=[C:2]1[NH:3][c:4]2[n:5][cH:6][cH:7][cH:8][c:9]2[CH2:10][N:11]1[CH:12]1[CH2:13][CH2:14][NH:15][CH2:16][CH2:17]1
O=C1Nc2ncccc2CN1C1CCN(Cc2ccccc2)CC1
O=C1Nc2ncccc2CN1C1CCNCC1
null
[Pd]
CO
Deprotection
Hydrogenolysis of tertiary amines
cd3c1aa319cad45f383f17cc0b8bfc8337d7078d779f654933f9a447e64292a5
1c99dd446c0bf4ae872cd8df8de34955be195747c234e9f3c49f46d1de614f66
O=C1Nc2ncccc2CN1C1CCNCC1
[C:1]-[C:2]-[N;H0;D3;+0:3](-C-c1:c:c:c:c:c:1)-[C:4]-[C:5]>>[C:1]-[C:2]-[NH;D2;+0:3]-[C:4]-[C:5]
null
[]
null
null
null
null
A solution of 4.7 g (0.0146 mol) of 3,4-dihydro-3-[1-(phenylmethyl)-4-piperidinyl]-2(1H)-pyrido[2,3-d]-pyrimidinone in 50 ml of methanol was hydrogenated at a temperature of 50° C. and in the presence of 2.0 g of 20% palladium/charcoal until the uptake of hydrogen ceased. After removal of the catalyst and solvent 3.3 g...
10.6084/m9.figshare.5104873.v1
null
Tertiary amine
Secondary amine
c1ccccc1.C1CC[NH]CC1
C1CCNCC1
c1cnc2c(c1)C[NH]CN2.C1CCNCC1
Other
[Pd].CO
null
null
O=C1Nc2ncccc2CN1C1CCN(Cc2ccccc2)CC1>[Pd].CO>O=C1Nc2ncccc2CN1C1CCNCC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e2c2cf6c7ccf4edbbce9fe82df963a88
COC(=O)c1ccc(C)c([N+](=O)[O-])c1.COC(OC)N(C)C>>COC(=O)c1ccc(/C=C/N(C)C)c([N+](=O)[O-])c1
CC1=C(C=C(C(=O)OC)C=C1)[N+](=O)[O-].COC(N(C)C)OC>>CN(\C=C\C1=C(C=C(C=C1)C(=O)OC)[N+](=O)[O-])C
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([CH3:9])[c:14]([N+:15](=[O:16])[O-:17])[cH:18]1.CO[CH:10](OC)[N:11]([CH3:12])[CH3:13]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8](/[CH:9]=[CH:10]/[N:11]([CH3:12])[CH3:13])[c:14]([N+:15](=[O:16])[O-:17])[cH:18]1
COC(=O)c1ccc(C)c([N+](=O)[O-])c1.COC(OC)N(C)C
COC(=O)c1ccc(/C=C/N(C)C)c([N+](=O)[O-])c1
null
null
CN(C=O)C
C-C Coupling
OtherReaction
83af34be484ee7162f3917cbabe10b671ad3f0d9bc6950031ada8dde2656d2d8
cd2513a82ead55986b41bf6d9bf4ca65c678444c433e242d0b640f08804ca4c6
c1ccccc1
C-O-[CH;D3;+0:1](-O-C)-[#7:2](-[C;D1;H3:3])-[C;D1;H3:4].[CH3;D1;+0:5]-[c:6](:[c:7]):[c:8]>>[C;D1;H3:3]-[#7:2](-[C;D1;H3:4])/[CH;D2;+0:1]=[CH;D2;+0:5]/[c:6](:[c:7]):[c:8]
null
[]
140
CELSIUS
null
null
A mixture of 98.3 g (0.504 mol) of methyl 4-methyl-3-nitrobenzoate, 78.0 g (0.655 mol) of N,N-dimethylformamide dimethylacetal and 1 l of dimethylformamide was heated to 140° C. for 3 hours. The solvent was distilled off in vacuo, the residue was triturated thoroughly with 1 l methanol. After drying in vacuo 119.5 g (9...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether
Enamine
null
null
c1ccccc1
HO-
CN(C=O)C
140
null
COC(=O)c1ccc(C)c([N+](=O)[O-])c1.COC(OC)N(C)C>CN(C=O)C>COC(=O)c1ccc(/C=C/N(C)C)c([N+](=O)[O-])c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8f43393d6a1145668204b71ffdc0ca52
COC(=O)c1ccc(/C=C/N(C)C)c([N+](=O)[O-])c1.[O-][I+3]([O-])([O-])[O-]>>COC(=O)c1ccc(C=O)c([N+](=O)[O-])c1
CN(\C=C\C1=C(C=C(C=C1)C(=O)OC)[N+](=O)[O-])C.I(=O)(=O)(=O)[O-].[Na+]>>COC(=O)C1=CC(=C(C=O)C=C1)[N+](=O)[O-]
CN(C)/C=[CH:9]/[c:8]1[cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:15][c:11]1[N+:12](=[O:13])[O-:14].[O-][I+3]([O-])([O-])[O-:10]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([CH:9]=[O:10])[c:11]([N+:12](=[O:13])[O-:14])[cH:15]1
COC(=O)c1ccc(/C=C/N(C)C)c([N+](=O)[O-])c1.[O-][I+3]([O-])([O-])[O-]
COC(=O)c1ccc(C=O)c([N+](=O)[O-])c1
null
null
O.O1CCCC1
Heteroatom Alkylation and Arylation
OtherReaction
1bc53144aaaadfebb6804333b37b20e33a34fa620575111a961d81231c604008
ee34f37ac54cbb3add9bb610747eeab45d01320a19fe84bf63f0866779dc68a8
c1ccccc1
C-N(-C)/C=[CH;D2;+0:1]/[c:2](:[c:3]):[c:4].[O-;H0;D1:5]-[I+3](-[O-])(-[O-])-[O-]>>[O;H0;D1;+0:5]=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
2.5
HOUR
To a mixture of 119.5 g (0.478 mol) of (E)-1-(dimethylamino)-2-[4-(methoxycarbonyl)-2-nitrophenyl]-ethene and 1.3 l of water/tetrahydrofuran mixture (1/1 v/v) were added, in batches, 308.0 g (1.44 mol) of sodium metaperiodate, whilst the reaction temperature was regulated at under +30° C. by external cooling with ice w...
10.6084/m9.figshare.5104873.v1
null
Enamine
Aldehyde
null
null
c1ccccc1
HI
O.O1CCCC1
null
2.5
COC(=O)c1ccc(/C=C/N(C)C)c([N+](=O)[O-])c1.[O-][I+3]([O-])([O-])[O-]>O.O1CCCC1>COC(=O)c1ccc(C=O)c([N+](=O)[O-])c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4491907cb0f14f1cb199fb1f36d8dd47
COC(=O)c1ccc(C=O)c([N+](=O)[O-])c1.NC1CCN(Cc2ccccc2)CC1>>COC(=O)c1ccc(CNC2CCN(Cc3ccccc3)CC2)c([N+](=O)[O-])c1
NC1CCN(CC1)CC1=CC=CC=C1.COC(=O)C1=CC(=C(C=O)C=C1)[N+](=O)[O-].[BH4-].[Na+]>>C1(=CC=CC=C1)CN1CCC(CC1)NCC1=C(C=C(C(=O)OC)C=C1)[N+](=O)[O-]
O=[CH:9][c:8]1[cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:28][c:24]1[N+:25](=[O:26])[O-:27].[NH2:10][CH:11]1[CH2:12][CH2:13][N:14]([CH2:15][c:16]2[cH:17][cH:18][cH:19][cH:20][cH:21]2)[CH2:22][CH2:23]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([CH2:9][NH:10][CH:11]2[CH2:12][CH2:13][N:14]([CH2:15][c:16]3[cH:1...
COC(=O)c1ccc(C=O)c([N+](=O)[O-])c1.NC1CCN(Cc2ccccc2)CC1
COC(=O)c1ccc(CNC2CCN(Cc3ccccc3)CC2)c([N+](=O)[O-])c1
null
null
CO
Functional Group Addition
Reductive amination with aldehyde
d42fc338dbdae89d3c539bd9d12d3b5ac50c40ef3b87bdc4c4d930c8ee74fb7d
b4dd31b60400cab3abb24376ebe2822f4ce30c85b6d3b9ac994d7e3c5f2bfd96
c1ccc(CNC2CCN(Cc3ccccc3)CC2)cc1
O=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4].[C:5]-[C:6](-[NH2;D1;+0:7])-[C:8]>>[C:5]-[C:6](-[NH;D2;+0:7]-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4])-[C:8]
null
[]
null
null
null
null
To a solution of 41.0 g (0.215 mol) of 4-amino-1-(phenylmethyl)-piperidine and 45.0 g (0.215 mol) of 4-(methoxycarbonyl)-2-nitrobenzaldehyde in 1 l methanol were added in batches, at room temperature, 8.3 g (0.22 mol) of sodium borohydride and the mixture was then stirred for 30 minutes at the same temperature. The mix...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary amine
Secondary amine
null
null
c1ccccc1.C1CC[NH]CC1.c1ccccc1
Other
CO
null
null
COC(=O)c1ccc(C=O)c([N+](=O)[O-])c1.NC1CCN(Cc2ccccc2)CC1>CO>COC(=O)c1ccc(CNC2CCN(Cc3ccccc3)CC2)c([N+](=O)[O-])c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-afcea6d8e8ac4fc7834c61852ba74c2f
COC(=O)c1ccc(CNC2CCN(Cc3ccccc3)CC2)c([N+](=O)[O-])c1>>COC(=O)c1ccc(CNC2CCN(Cc3ccccc3)CC2)c(N)c1
C1(=CC=CC=C1)CN1CCC(CC1)NCC1=C(C=C(C(=O)OC)C=C1)[N+](=O)[O-]>>NC=1C=C(C(=O)OC)C=CC1CNC1CCN(CC1)CC1=CC=CC=C1
O=[N+:25]([O-])[c:24]1[c:8]([CH2:9][NH:10][CH:11]2[CH2:12][CH2:13][N:14]([CH2:15][c:16]3[cH:17][cH:18][cH:19][cH:20][cH:21]3)[CH2:22][CH2:23]2)[cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:26]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([CH2:9][NH:10][CH:11]2[CH2:12][CH2:13][N:14]([CH2:15][c:16]3[cH:17][cH:18]...
COC(=O)c1ccc(CNC2CCN(Cc3ccccc3)CC2)c([N+](=O)[O-])c1
COC(=O)c1ccc(CNC2CCN(Cc3ccccc3)CC2)c(N)c1
null
[Rh].C
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc(CNC2CCN(Cc3ccccc3)CC2)cc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
A solution of 58.0 g (0.151 mol) of methyl 4-[[[1-(phenylmethyl)-4-piperidinyl]amino]methyl]-3-nitrobenzoate in 800 ml of methanol was hydrogenated in the presence of 10 g of 5% rhodium/charcoal for 7 hours at room temperature. The catalyst was filtered off, the filtrate was evaporated down in vacuo. 50.0 g (93.7% of t...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1.C1CC[NH]CC1.c1ccccc1
Other
[Rh].C.CO
null
null
COC(=O)c1ccc(CNC2CCN(Cc3ccccc3)CC2)c([N+](=O)[O-])c1>[Rh].C.CO>COC(=O)c1ccc(CNC2CCN(Cc3ccccc3)CC2)c(N)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4dee884051634d85978fb60409e5c8dd
CCOC(=O)Cl.COC(=O)c1cscc1N>>CCOC(=O)Nc1cscc1C(=O)OC
Cl.NC=1C(=CSC1)C(=O)OC.C(C)N(CC)CC.C(OCC)(=O)Cl>>C(C)OC(=O)NC=1C(=CSC1)C(=O)OC
Cl[C:4]([O:3][CH2:2][CH3:1])=[O:5].[NH2:6][c:7]1[cH:8][s:9][cH:10][c:11]1[C:12](=[O:13])[O:14][CH3:15]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[NH:6][c:7]1[cH:8][s:9][cH:10][c:11]1[C:12](=[O:13])[O:14][CH3:15]
CCOC(=O)Cl.COC(=O)c1cscc1N
CCOC(=O)Nc1cscc1C(=O)OC
null
null
C1(=CC=CC=C1)C
Protection
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
038720aa61a7efa0f2a9ee6f2e0adf63a9ffdc2be4697c11a6215baef34f97b2
205f353513ce9506ab61831799da8fb73ec2ef5cfa927664496d3ce72c438860
c1ccsc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C:4].[#8:5]-[C:6](=[O;D1;H0:7])-[c:8]1:[c:9]:[#16;a:10]:[c:11]:[c:12]:1-[NH2;D1;+0:13]>>[#8:5]-[C:6](=[O;D1;H0:7])-[c:8]1:[c:9]:[#16;a:10]:[c:11]:[c:12]:1-[NH;D2;+0:13]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C:4]
null
[]
null
null
null
null
A mixture of 50.0 g (0.258 mol) of methyl 4-aminothiophen-3-carboxylate-hydrochloride, 700 ml of toluene, 26 g (0.257 mol) of triethylamine and 27 ml (0.283 mol) of ethyl chlorocarbonate was refluxed for 5 hours. The insoluble matter was filtered off, the filtrate was evaporated down in vacuo and the residue was crysta...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Ether.Primary amine
Carbamic ester
null
null
c1ccsc1
HCl
C1(=CC=CC=C1)C
null
null
CCOC(=O)Cl.COC(=O)c1cscc1N>C1(=CC=CC=C1)C>CCOC(=O)Nc1cscc1C(=O)OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-12cfe412697a4cd0af7243a718237d05
CCOC(=O)Nc1cscc1C(=O)OC>>CCOC(=O)Nc1cscc1C=O
[H-].[Al+3].[Li+].[H-].[H-].[H-].C(C)OC(=O)NC=1C(=CSC1)C(=O)OC.O.[OH-].[Na+].O>>C(C)OC(=O)NC=1C(=CSC1)C=O
CO[C:12]([c:11]1[c:7]([NH:6][C:4]([O:3][CH2:2][CH3:1])=[O:5])[cH:8][s:9][cH:10]1)=[O:13]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[NH:6][c:7]1[cH:8][s:9][cH:10][c:11]1[CH:12]=[O:13]
CCOC(=O)Nc1cscc1C(=O)OC
CCOC(=O)Nc1cscc1C=O
null
null
C(C)(C)(C)OC
Reduction
OtherReaction
ec1c6c64dd9be73981e5a6c952ab740869d298b20e87e097e88e1179cc5bc6dc
33ddc7b9457742ba0a376f08a972e4f33779267f6f1fe15e3be786427ae9f4ec
c1ccsc1
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#16;a:5]:[c:6]:[c:7]:1>>[O;D1;H0:2]=[CH;D2;+0:1]-[c:3]1:[c:4]:[#16;a:5]:[c:6]:[c:7]:1
null
[]
null
null
1
HOUR
Into an ice-cold suspension of 12.9 g (0.34 mol) of lithium aluminium hydride in 800 ml of tert. butyl-methylether was added dropwise, at a reaction temperature of about 0° C., a solution of 59.1 g (0.258 mol) of methyl 4-(ethoxycarbonylamino)-thiophene-3-carboxylate in 200 ml of tert. butyl-methylether, and the mixtur...
10.6084/m9.figshare.5104873.v1
null
Ester
Aldehyde
null
null
c1ccsc1
HO-
C(C)(C)(C)OC
null
1
CCOC(=O)Nc1cscc1C(=O)OC>C(C)(C)(C)OC>CCOC(=O)Nc1cscc1C=O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2bc2df2cc74f40edba51ff4f322dc1db
CC(C)(C)OC(=O)N1CCC(N)CC1.CCOC(=O)Nc1cscc1C=O>>CCOC(=O)Nc1cscc1CNC1CCN(C(=O)OC(C)(C)C)CC1
[BH4-].[Na+].C(C)OC(=O)NC=1C(=CSC1)C=O.NC1CCN(CC1)C(=O)OC(C)(C)C.C1(=CC=CC=C1)C>>CC(C)(OC(=O)N1CCC(CC1)NCC=1C(=CSC1)NC(=O)OCC)C
[NH2:13][CH:14]1[CH2:15][CH2:16][N:17]([C:18](=[O:19])[O:20][C:21]([CH3:22])([CH3:23])[CH3:24])[CH2:25][CH2:26]1.O=[CH:12][c:11]1[c:7]([NH:6][C:4]([O:3][CH2:2][CH3:1])=[O:5])[cH:8][s:9][cH:10]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[NH:6][c:7]1[cH:8][s:9][cH:10][c:11]1[CH2:12][NH:13][CH:14]1[CH2:15][CH2:16][N:17]([C:18](=[O...
CC(C)(C)OC(=O)N1CCC(N)CC1.CCOC(=O)Nc1cscc1C=O
CCOC(=O)Nc1cscc1CNC1CCN(C(=O)OC(C)(C)C)CC1
null
null
O
Heteroatom Alkylation and Arylation
Reductive amination with aldehyde
422be648aea52bce28ccc8fb32ec3178aaa47bbd624f063874619362f075b5f2
7915721a3e395aed85e3c40dc4d725c571a931ac517c6a0da16f2a2b0bb5eac7
c1cc(CNC2CCNCC2)cs1
O=[CH;D2;+0:1]-[c:2]1:[c:3]:[#16;a:4]:[c:5]:[c:6]:1.[C:7]-[C:8](-[NH2;D1;+0:9])-[C:10]>>[C:7]-[C:8](-[NH;D2;+0:9]-[CH2;D2;+0:1]-[c:2]1:[c:3]:[#16;a:4]:[c:5]:[c:6]:1)-[C:10]
null
[]
null
null
null
null
A mixture of 28.2 g (0.142 mol) of 4-(ethoxycarbonyl-amino)-thiophene-3-carboxaldehyde, 28.2 g (0.141 mol) of 4-amino-1-(1,1-dimethyl-ethoxycarbonyl)piperidine and 300 ml of toluene was refluxed using a water separator until water formation had ceased. The solvent was removed in vacuo, the residue was dissolved in 300 ...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary amine
Secondary amine
null
null
c1ccsc1.C1CC[NH]CC1
Other
O
null
null
CC(C)(C)OC(=O)N1CCC(N)CC1.CCOC(=O)Nc1cscc1C=O>O>CCOC(=O)Nc1cscc1CNC1CCN(C(=O)OC(C)(C)C)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e7a875b97ebe4b8d8c79a2571fbe561e
CC(C)(C)OC(=O)N1CCC(N2Cc3cscc3NC2=O)CC1.O=C(O)C(F)(F)F>>O=C([O-])C(F)(F)F.O=C1Nc2cscc2CN1C1CCNCC1
CC(C)(OC(=O)N1CCC(CC1)N1C(NC=2C(C1)=CSC2)=O)C.FC(C(=O)O)(F)F>>N1CCC(CC1)N1C(NC=2C(C1)=CSC2)=O.FC(C(=O)[O-])(F)F
CC(C)(C)OC(=O)[N:21]1[CH2:20][CH2:19][CH:18]([N:17]2[C:9](=[O:8])[NH:10][c:11]3[cH:12][s:13][cH:14][c:15]3[CH2:16]2)[CH2:23][CH2:22]1.[O:1]=[C:2]([OH:3])[C:4]([F:5])([F:6])[F:7]>>[O:1]=[C:2]([O-:3])[C:4]([F:5])([F:6])[F:7].[O:8]=[C:9]1[NH:10][c:11]2[cH:12][s:13][cH:14][c:15]2[CH2:16][N:17]1[CH:18]1[CH2:19][CH2:20][NH:2...
CC(C)(C)OC(=O)N1CCC(N2Cc3cscc3NC2=O)CC1.O=C(O)C(F)(F)F
O=C([O-])C(F)(F)F.O=C1Nc2cscc2CN1C1CCNCC1
null
null
null
Miscellaneous
OtherReaction
682e089fbfc4d16c974a525961e4df91784d114b83c27ef342a0481baecd0ade
3b21d7a593211fb542228e23c12b5c46779cf3cdc7f54f93350e1b43ee65b9f4
O=C1Nc2cscc2CN1C1CCNCC1
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1](-[C:2]-[C:3])-[C:4]-[C:5].[F;D1;H0:6]-[C:7](-[F;D1;H0:8])(-[F;D1;H0:9])-[C:10](=[O;D1;H0:11])-[OH;D1;+0:12]>>[C:3]-[C:2]-[NH;D2;+0:1]-[C:4]-[C:5].[F;D1;H0:6]-[C:7](-[F;D1;H0:8])(-[F;D1;H0:9])-[C:10](-[O-;H0;D1:12])=[O;D1;H0:11]
null
[]
null
null
30
MINUTE
A mixture of 10.0 g (0.0296 mol) of 3,4-dihydro-3-[1-(1,1-dimethylethoxycarbonyl)-4-piperidinyl]-1H-thieno[3,4-d]pyrimidin-2-one and 50 ml of trifluoroacetic acid was stirred at room temperature for 30 minutes. The residue remaining after removal of the excess trifluoroacetic acid was triturated with diethylether and s...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Carboxylic acid.Ether.Boc
Secondary amine
C1CC[NH]CC1
C1CCNCC1
c1scc2c1C[NH]CN2.C1CCNCC1
HO-
null
null
0.5
CC(C)(C)OC(=O)N1CCC(N2Cc3cscc3NC2=O)CC1.O=C(O)C(F)(F)F>>O=C([O-])C(F)(F)F.O=C1Nc2cscc2CN1C1CCNCC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-87cef751482546b88fce41513d644f7c
O=c1[nH]c2ccccc2cc1-c1ccncc1>>O=C1Nc2ccccc2CC1C1CCNCC1
N1=CC=C(C=C1)C=1C(NC2=CC=CC=C2C1)=O.Cl>>Cl.N1CCC(CC1)C1C(NC2=CC=CC=C2C1)=O
[O:2]=[c:3]1[nH:4][c:5]2[cH:6][cH:7][cH:8][cH:9][c:10]2[cH:11][c:12]1-[c:13]1[cH:14][cH:15][n:16][cH:17][cH:18]1>>[O:2]=[C:3]1[NH:4][c:5]2[cH:6][cH:7][cH:8][cH:9][c:10]2[CH2:11][CH:12]1[CH:13]1[CH2:14][CH2:15][NH:16][CH2:17][CH2:18]1
O=c1[nH]c2ccccc2cc1-c1ccncc1
O=C1Nc2ccccc2CC1C1CCNCC1
null
[Pt](=O)=O
C(C)O
Reduction
OtherReaction
338a6fd42b5469849527cb5dc5a3275784c739143a9f5003b69ee45ab7cbf4b8
211104e8b119db7b18ca563982f63840af02165e5ca58709899a446d5754a027
O=C1Nc2ccccc2CC1C1CCNCC1
[O;D1;H0:1]=[c;H0;D3;+0:2]1:[nH;D2;+0:3]:[c:4](:[c:5]):[c:6](:[c:7]):[cH;D2;+0:8]:[c;H0;D3;+0:9]:1-[c;H0;D3;+0:10]1:[cH;D2;+0:11]:[cH;D2;+0:12]:[n;H0;D2;+0:13]:[cH;D2;+0:14]:[cH;D2;+0:15]:1>>[O;D1;H0:1]=[C;H0;D3;+0:2]1-[NH;D2;+0:3]-[c:4](:[c:5]):[c:6](:[c:7])-[CH2;D2;+0:8]-[CH;D3;+0:9]-1-[CH;D3;+0:10]1-[CH2;D2;+0:11]-[...
null
[]
null
null
4
HOUR
A mixture of 1.1 g (4.949 mmol) of 3-(4-pyridinyl)-2(1H)-quinolone (D. R. Bragg and D. G. Wibberley, J. Chem. Soc. 1961, 5074-5077), 100 ml of ethanol, 5 ml (5 mmol) of 1N hydrochloric acid and 0.2 g platinum (IV) oxide was hydrogenated for 4 hours at room temperature. The catalyst was filtered off, the filtrate evapor...
10.6084/m9.figshare.5104873.v1
null
null
Secondary amide.Secondary amine
c1cnc2ccccc2c1.c1ccncc1
c1ccc2c(c1)CCCN2.C1CCNCC1
c1ccc2c(c1)CCCN2.C1CCNCC1
null
[Pt](=O)=O.C(C)O
null
4
O=c1[nH]c2ccccc2cc1-c1ccncc1>[Pt](=O)=O.C(C)O>O=C1Nc2ccccc2CC1C1CCNCC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c7ba1bc8ae2e46cf9c66cbd38f66d461
O=c1[nH]c2ccccc2cc1-c1ccncc1>>O=c1cc(N2CCCCC2)c2ccccc2[nH]1
N1=CC=C(C=C1)C=1C(NC2=CC=CC=C2C1)=O.Cl.[H][H]>>N1(CCCCC1)C1=CC(NC2=CC=CC=C12)=O
[O:1]=[c:2]1[c:3](-[c:8]2[cH:7][cH:6][n:5][cH:9][cH:10]2)[cH:4][c:11]2[cH:12][cH:13][cH:14][cH:15][c:16]2[nH:17]1>>[O:1]=[c:2]1[cH:3][c:4]([N:5]2[CH2:6][CH2:7][CH2:8][CH2:9][CH2:10]2)[c:11]2[cH:12][cH:13][cH:14][cH:15][c:16]2[nH:17]1
O=c1[nH]c2ccccc2cc1-c1ccncc1
O=c1cc(N2CCCCC2)c2ccccc2[nH]1
null
[Pd]
C(C)O
Miscellaneous
OtherReaction
83903bfe79e2b2f0bc9f5438967ab0682e7e694b8433de0ac04c44b9bd87cae2
4c812c1c920bf53b5923291709d187e223e40a94df3acb57982c9a7523919d2a
O=c1cc(N2CCCCC2)c2ccccc2[nH]1
[O;D1;H0:1]=[c:2]1:[#7;a:3]:[c:4](:[c:5]):[c:6](:[c:7]):[cH;D2;+0:8]:[c;H0;D3;+0:9]:1-[c;H0;D3;+0:10]1:[cH;D2;+0:11]:[cH;D2;+0:12]:[n;H0;D2;+0:13]:[cH;D2;+0:14]:[cH;D2;+0:15]:1>>[O;D1;H0:1]=[c:2]1:[#7;a:3]:[c:4](:[c:5]):[c:6](:[c:7]):[c;H0;D3;+0:8](-[N;H0;D3;+0:13]2-[CH2;D2;+0:11]-[CH2;D2;+0:12]-[CH2;D2;+0:10]-[CH2;D2;...
null
[]
null
null
null
null
A mixture of 8.6 g (0.0387 mol) of 3-(4-pyridinyl)-2(1H)-quinolone, 1.2 l of ethanol, 39 ml (0.039 mol) of 1N hydrochloric acid and 8.0 g of 10% palladium/charcoal was hydrogenated at a temperature of 40° C. until about 0.08 mol of hydrogen had been taken up. The mixture was freed from catalyst, the filtrate was evapor...
10.6084/m9.figshare.5104873.v1
null
null
Tertiary amine
c1ccncc1.c1cnc2ccccc2c1
C1CC[NH]CC1.c1ccc2ccccc2n1
C1CC[NH]CC1.c1ccc2ccccc2n1
null
[Pd].C(C)O
null
null
O=c1[nH]c2ccccc2cc1-c1ccncc1>[Pd].C(C)O>O=c1cc(N2CCCCC2)c2ccccc2[nH]1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-71b9ae1165ef4c35902a8fb64b852509
O=C1Nc2cccc(Cl)c2CN1C1CCN(Cc2ccccc2)CC1>>O=C1Nc2cccc(Cl)c2CN1C1CCNCC1
ClC1=C2CN(C(NC2=CC=C1)=O)C1CCN(CC1)CC1=CC=CC=C1.C(OC(C)Cl)(=O)Cl>>ClC1=C2CN(C(NC2=CC=C1)=O)C1CCNCC1
c1ccc(C[N:16]2[CH2:15][CH2:14][CH:13]([N:12]3[C:2](=[O:1])[NH:3][c:4]4[cH:5][cH:6][cH:7][c:8]([Cl:9])[c:10]4[CH2:11]3)[CH2:18][CH2:17]2)cc1>>[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][cH:7][c:8]([Cl:9])[c:10]2[CH2:11][N:12]1[CH:13]1[CH2:14][CH2:15][NH:16][CH2:17][CH2:18]1
O=C1Nc2cccc(Cl)c2CN1C1CCN(Cc2ccccc2)CC1
O=C1Nc2cccc(Cl)c2CN1C1CCNCC1
null
null
ClCCl
Deprotection
Hydrogenolysis of tertiary amines
cd3c1aa319cad45f383f17cc0b8bfc8337d7078d779f654933f9a447e64292a5
1c99dd446c0bf4ae872cd8df8de34955be195747c234e9f3c49f46d1de614f66
O=C1Nc2ccccc2CN1C1CCNCC1
[C:1]-[C:2]-[N;H0;D3;+0:3](-C-c1:c:c:c:c:c:1)-[C:4]-[C:5]>>[C:1]-[C:2]-[NH;D2;+0:3]-[C:4]-[C:5]
null
[]
0
CELSIUS
null
null
An ice-cold solution of 6.3 g (0.0177 mol) of 5-chloro-3,4-dihydro-3-[1-(phenylmethyl)-4-piperidinyl]-2(1H)-quinazolinone (prepared analogously to Example A4e)) in 50 ml of dichloromethane was mixed dropwise with 3.34 g (0.0234 mol) of (α-chloroethyl chlorocarbonate whilst maintaining a reaction temperature of 0° C., a...
10.6084/m9.figshare.5104873.v1
null
Tertiary amine
Secondary amine
c1ccccc1.C1CC[NH]CC1
C1CCNCC1
c1ccc2c(c1)C[NH]CN2.C1CCNCC1
Other
ClCCl
0
null
O=C1Nc2cccc(Cl)c2CN1C1CCN(Cc2ccccc2)CC1>ClCCl>O=C1Nc2cccc(Cl)c2CN1C1CCNCC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-de5f82b46ecb4eeab685bf270778f146
BrBr.O=C1Nc2ccccc2CN1C1CCNCC1>>Br.O=C1Nc2ccc(Br)cc2CN1C1CCNCC1
C(C)(=O)[O-].[Na+].N1CCC(CC1)N1C(NC2=CC=CC=C2C1)=O.BrBr>>Br.BrC=1C=C2CN(C(NC2=CC1)=O)C1CCNCC1
[Br:1][Br:9].[O:2]=[C:3]1[NH:4][c:5]2[cH:6][cH:7][cH:8][cH:10][c:11]2[CH2:12][N:13]1[CH:14]1[CH2:15][CH2:16][NH:17][CH2:18][CH2:19]1>>[BrH:1].[O:2]=[C:3]1[NH:4][c:5]2[cH:6][cH:7][c:8]([Br:9])[cH:10][c:11]2[CH2:12][N:13]1[CH:14]1[CH2:15][CH2:16][NH:17][CH2:18][CH2:19]1
BrBr.O=C1Nc2ccccc2CN1C1CCNCC1
Br.O=C1Nc2ccc(Br)cc2CN1C1CCNCC1
null
null
O.C(C)(=O)O
Miscellaneous
Bromination
62ade74d96be9803b859f68bffbf6b388ebc22ac2e4b4efe0e6f817cee0cb193
a48150e9dff88baab32dd83daf5ab089c597626e3c583c33a5868d8e1353c1ea
O=C1Nc2ccccc2CN1C1CCNCC1
[Br;H0;D1;+0:1]-[Br;H0;D1;+0:2].[c:3]:[c:4]:[cH;D2;+0:5]:[c:6]:[c:7]>>[Br;H0;D1;+0:2]-[c;H0;D3;+0:5](:[c:4]:[c:3]):[c:6]:[c:7].[BrH;D0;+0:1]
null
[]
14
CELSIUS
null
null
To a solution of 6.16 g (0.075 mol) of sodium acetate and 11.565 g (0.05 mol) of 3,4-dihydro-3-(4-piperidinyl)-2(1H)-quinazolinone in a mixture of 150 ml of glacial acetic acid and 35 ml of water a solution of 8.8 g (0.055 mol) of anhydrous bromine in 20 ml of glacial acetic acid was added dropwise, with stirring and w...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2c(c1)C[NH]CN2
c1ccc2c(c1)C[NH]CN2
c1ccc2c(c1)C[NH]CN2.C1CCNCC1
null
O.C(C)(=O)O
14
null
BrBr.O=C1Nc2ccccc2CN1C1CCNCC1>O.C(C)(=O)O>Br.O=C1Nc2ccc(Br)cc2CN1C1CCNCC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6db817171436441985f094ec712656cc
NC1CCN(Cc2ccccc2)CC1.O=c1[nH]c2ccccc2c(=O)o1>>Nc1ccccc1C(=O)NC1CCN(Cc2ccccc2)CC1
NC1CCN(CC1)CC1=CC=CC=C1.C1=2C(=O)OC(NC1=CC=CC2)=O>>NC1=C(C(=O)NC2CCN(CC2)CC2=CC=CC=C2)C=CC=C1
[NH2:10][CH:11]1[CH2:12][CH2:13][N:14]([CH2:15][c:16]2[cH:17][cH:18][cH:19][cH:20][cH:21]2)[CH2:22][CH2:23]1.O=c1o[c:8](=[O:9])[c:7]2[c:2]([nH:1]1)[cH:3][cH:4][cH:5][cH:6]2>>[NH2:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1[C:8](=[O:9])[NH:10][CH:11]1[CH2:12][CH2:13][N:14]([CH2:15][c:16]2[cH:17][cH:18][cH:19][cH:20][cH:21]2)...
NC1CCN(Cc2ccccc2)CC1.O=c1[nH]c2ccccc2c(=O)o1
Nc1ccccc1C(=O)NC1CCN(Cc2ccccc2)CC1
null
null
O1CCCC1.C(C)O
Acylation
OtherReaction
05f2f4b560cbf584ccb0bd125cb5ac7db8ee3251741e8cf30be7edbfdf8b694e
b609a70ccab739990a9ccc4ea2adcc77011bcd0c07154489a12420f7c0e7382e
O=C(NC1CCN(Cc2ccccc2)CC1)c1ccccc1
O=c1:[nH;D2;+0:1]:[c:2](:[c:3]):[c:4](:[c:5]):[c;H0;D3;+0:6](=[O;D1;H0:7]):o:1.[C:8]-[C:9](-[NH2;D1;+0:10])-[C:11]>>[C:8]-[C:9](-[NH;D2;+0:10]-[C;H0;D3;+0:6](=[O;D1;H0:7])-[c:4](:[c:5]):[c:2](-[NH2;D1;+0:1]):[c:3])-[C:11]
68.3
[{"value": 68.3, "product": "NC1=C(C(=O)NC2CCN(CC2)CC2=CC=CC=C2)C=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To an ice-cold solution of 28 ml (134 mmol) of 4-amino-1-(phenylmethyl)piperidine in 200 ml of tetrahydrofuran were added, batchwise, 21.9 g (134 mmol) of isatoic acid anhydride. The resulting suspension was stirred for 2½ hours at room temperature and 2½ hours at reflux temperature, then freed from solvent. The residu...
10.6084/m9.figshare.5104873.v1
null
Primary amine
Secondary amide.Primary amine
c1ocnc2ccccc12
c1ccccc1
c1ccccc1.C1CC[NH]CC1.c1ccccc1
Other
O1CCCC1.C(C)O
null
null
NC1CCN(Cc2ccccc2)CC1.O=c1[nH]c2ccccc2c(=O)o1>O1CCCC1.C(C)O>Nc1ccccc1C(=O)NC1CCN(Cc2ccccc2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-87a01a56e7674e36a17dab6713efaf0a
O=C1Nc2ccccc2CN1C1CCN(C2CCN(Cc3ccccc3)CC2)CC1>>O=C1Nc2ccccc2CN1C1CCN(C2CCNCC2)CC1
C1(=CC=CC=C1)CN1CCC(CC1)N1CCC(CC1)N1C(NC2=CC=CC=C2C1)=O.N>>N1CCC(CC1)N1CCC(CC1)N1C(NC2=CC=CC=C2C1)=O
c1ccc(C[N:19]2[CH2:18][CH2:17][CH:16]([N:15]3[CH2:14][CH2:13][CH:12]([N:11]4[C:2](=[O:1])[NH:3][c:4]5[cH:5][cH:6][cH:7][cH:8][c:9]5[CH2:10]4)[CH2:23][CH2:22]3)[CH2:21][CH2:20]2)cc1>>[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2[CH2:10][N:11]1[CH:12]1[CH2:13][CH2:14][N:15]([CH:16]2[CH2:17][CH2:18][NH:19][CH2:20...
O=C1Nc2ccccc2CN1C1CCN(C2CCN(Cc3ccccc3)CC2)CC1
O=C1Nc2ccccc2CN1C1CCN(C2CCNCC2)CC1
null
[OH-].[OH-].[Pd+2]
ClCCl.CO.C1CCCCC1
Deprotection
Hydrogenolysis of tertiary amines
cd3c1aa319cad45f383f17cc0b8bfc8337d7078d779f654933f9a447e64292a5
1c99dd446c0bf4ae872cd8df8de34955be195747c234e9f3c49f46d1de614f66
O=C1Nc2ccccc2CN1C1CCN(C2CCNCC2)CC1
[C:1]-[C:2]-[N;H0;D3;+0:3](-C-c1:c:c:c:c:c:1)-[C:4]-[C:5]>>[C:1]-[C:2]-[NH;D2;+0:3]-[C:4]-[C:5]
92
[{"value": 92.0, "product": "N1CCC(CC1)N1CCC(CC1)N1C(NC2=CC=CC=C2C1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
Prepared analogously to Example A3f) from 3,4-dihydro-3-[1-[1-(phenylmethyl)-4-piperidinyl]-4-piperidinyl]-2(1H)-quinazolinone by hydrogenolysis, but using Pearlman's catalyst, in a yield of 92% of theory. Colourless crystals, Rf=0.48 (Macherey-Nagel, POLYGRAM® SIL G/UV254ready-made films for TLC; eluant: dichlorometha...
10.6084/m9.figshare.5104873.v1
null
Tertiary amine
Secondary amine
c1ccccc1.C1CC[NH]CC1
C1CCNCC1
c1ccc2c(c1)C[NH]CN2.C1CC[NH]CC1.C1CCNCC1
Other
[OH-].[OH-].[Pd+2].ClCCl.CO.C1CCCCC1
null
null
O=C1Nc2ccccc2CN1C1CCN(C2CCN(Cc3ccccc3)CC2)CC1>[OH-].[OH-].[Pd+2].ClCCl.CO.C1CCCCC1>O=C1Nc2ccccc2CN1C1CCN(C2CCNCC2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c77a00f1f4914724b3abd5bbcc00f5e6
O=C1Nc2ccccc2CN1C1CCNCC1>>O=C1NC2CCCCC2CN1C1CCNCC1
N.[H][H].N1CCC(CC1)N1C(NC2=CC=CC=C2C1)=O.C(C)(=O)[O-].ClCCl.CO>>N1CCC(CC1)N1C(NC2CCCCC2C1)=O.C(C)(=O)[O-]
[O:5]=[C:6]1[NH:7][c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]2[CH2:14][N:15]1[CH:16]1[CH2:17][CH2:18][NH:19][CH2:20][CH2:21]1>>[O:5]=[C:6]1[NH:7][CH:8]2[CH2:9][CH2:10][CH2:11][CH2:12][CH:13]2[CH2:14][N:15]1[CH:16]1[CH2:17][CH2:18][NH:19][CH2:20][CH2:21]1
O=C1Nc2ccccc2CN1C1CCNCC1
O=C1NC2CCCCC2CN1C1CCNCC1
null
[Rh+]=O.O.[Pt](=O)=O
CO
Reduction
Arene hydrogenation
1246ee61807f1157c941c0c1d66e1757d2db4a83ff8514b6b86ee2a2e16cdf32
312e9350dcad67590617294c0eb017edf0b9fbfe6133c06a3f393b871a889092
O=C1NC2CCCCC2CN1C1CCNCC1
[C:1]-[#7:2]1-[C:3]-[c;H0;D3;+0:4]2:[cH;D2;+0:5]:[cH;D2;+0:6]:[cH;D2;+0:7]:[cH;D2;+0:8]:[c;H0;D3;+0:9]:2-[#7:10]-[C:11]-1=[O;D1;H0:12]>>[C:1]-[#7:2]1-[C:3]-[CH;D3;+0:4]2-[CH2;D2;+0:5]-[CH2;D2;+0:6]-[CH2;D2;+0:7]-[CH2;D2;+0:8]-[CH;D3;+0:9]-2-[#7:10]-[C:11]-1=[O;D1;H0:12]
null
[]
null
null
null
null
A solution of 5.0 g (17.17 mmol) of 3,4-dihydro-3-(4-piperidinyl)-2(1H)-quinazolinone-acetate in 70 ml of methanol was hydrogenated at room temperature and in the presence of 1.0 g rhodium (III) oxide-platinum (IV) oxide hydrate catalyst (46.45% rhodium, 20.15% platinum) until the hydrogen uptake had ceased. The cataly...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ccc2c(c1)C[NH]CN2
C1CCC2NC[NH]CC2C1
C1CCC2NC[NH]CC2C1.C1CCNCC1
null
[Rh+]=O.O.[Pt](=O)=O.CO
null
null
O=C1Nc2ccccc2CN1C1CCNCC1>[Rh+]=O.O.[Pt](=O)=O.CO>O=C1NC2CCCCC2CN1C1CCNCC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-fa4bb05d0c4c4347bdb647373b5eaf41
NC1CCN(Cc2ccccc2)CC1.O=[N+]([O-])c1ccccc1S(=O)(=O)Cl>>O=[N+]([O-])c1ccccc1S(=O)(=O)NC1CCN(Cc2ccccc2)CC1
[N+](=O)([O-])C1=C(C=CC=C1)S(=O)(=O)Cl.NC1CCN(CC1)CC1=CC=CC=C1.C(C)N(CC)CC>>[N+](=O)([O-])C1=C(C=CC=C1)S(=O)(=O)NC1CCN(CC1)CC1=CC=CC=C1
[NH2:13][CH:14]1[CH2:15][CH2:16][N:17]([CH2:18][c:19]2[cH:20][cH:21][cH:22][cH:23][cH:24]2)[CH2:25][CH2:26]1.Cl[S:10]([c:9]1[c:4]([N+:2](=[O:1])[O-:3])[cH:5][cH:6][cH:7][cH:8]1)(=[O:11])=[O:12]>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][cH:7][cH:8][c:9]1[S:10](=[O:11])(=[O:12])[NH:13][CH:14]1[CH2:15][CH2:16][N:17]([CH2:18...
NC1CCN(Cc2ccccc2)CC1.O=[N+]([O-])c1ccccc1S(=O)(=O)Cl
O=[N+]([O-])c1ccccc1S(=O)(=O)NC1CCN(Cc2ccccc2)CC1
null
null
C(Cl)(Cl)Cl
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=S(=O)(NC1CCN(Cc2ccccc2)CC1)c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[C:7]-[C:8](-[NH2;D1;+0:9])-[C:10]>>[C:7]-[C:8](-[NH;D2;+0:9]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6])-[C:10]
null
[]
null
null
30
MINUTE
Whilst carrying out external cooling with ice water a solution of 44.3 g (0.2 mol) of 2-nitrobenzenesulphonyl chloride in 250 ml of chloroform was added dropwise to a solution of 38.0 g (0.2 mol) of 4-amino-1-(phenylmethyl)piperidine and 22.0 g (0.22 mol) of triethylamine in 250 ml of chloroform. After the cooling was ...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccccc1.C1CC[NH]CC1.c1ccccc1
HCl
C(Cl)(Cl)Cl
null
0.5
NC1CCN(Cc2ccccc2)CC1.O=[N+]([O-])c1ccccc1S(=O)(=O)Cl>C(Cl)(Cl)Cl>O=[N+]([O-])c1ccccc1S(=O)(=O)NC1CCN(Cc2ccccc2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c16f0b3efb414c96b5009953046aea03
O=[N+]([O-])c1ccccc1S(=O)(=O)NC1CCN(Cc2ccccc2)CC1>>Nc1ccccc1S(=O)(=O)NC1CCN(Cc2ccccc2)CC1
[N+](=O)([O-])C1=C(C=CC=C1)S(=O)(=O)NC1CCN(CC1)CC1=CC=CC=C1.O.O.S(=O)([O-])S(=O)[O-].[Na+].[Na+]>>NC1=C(C=CC=C1)S(=O)(=O)NC1CCN(CC1)CC1=CC=CC=C1
O=[N+:1]([O-])[c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1[S:8](=[O:9])(=[O:10])[NH:11][CH:12]1[CH2:13][CH2:14][N:15]([CH2:16][c:17]2[cH:18][cH:19][cH:20][cH:21][cH:22]2)[CH2:23][CH2:24]1>>[NH2:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1[S:8](=[O:9])(=[O:10])[NH:11][CH:12]1[CH2:13][CH2:14][N:15]([CH2:16][c:17]2[cH:18][cH:19][cH:20]...
O=[N+]([O-])c1ccccc1S(=O)(=O)NC1CCN(Cc2ccccc2)CC1
Nc1ccccc1S(=O)(=O)NC1CCN(Cc2ccccc2)CC1
null
null
O.C(C)O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
O=S(=O)(NC1CCN(Cc2ccccc2)CC1)c1ccccc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
To a solution of 75.0 g (0.2 mol) of 2-nitro-N-[1-(phenylmethyl)-4-piperidinyl]-benzenesulphonic acid amide in 2.0 l ethanol was added dropwise, at room temperature, a solution of 174.0 g ( 0.828 mol) of sodium dithionite-dihydrate in 700 ml of water. After the heat of the exothermic reaction had died away the mixture ...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1.C1CC[NH]CC1.c1ccccc1
Other
O.C(C)O
null
null
O=[N+]([O-])c1ccccc1S(=O)(=O)NC1CCN(Cc2ccccc2)CC1>O.C(C)O>Nc1ccccc1S(=O)(=O)NC1CCN(Cc2ccccc2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-15fb64b0243f426eb0e8ea24464000af
NS(N)(=O)=O.Nc1ccccc1CNC1CCN(Cc2ccccc2)CC1>>O=S1(=O)Nc2ccccc2CN1C1CCN(Cc2ccccc2)CC1
NC1=C(C=CC=C1)CNC1CCN(CC1)CC1=CC=CC=C1.S(=O)(=O)(N)N>>O=S1(NC2=C(CN1C1CCN(CC1)CC1=CC=CC=C1)C=CC=C2)=O
N[S:2](=[O:1])(=[O:3])[NH2:4].N[c:5]1[cH:6][cH:7][cH:8][cH:9][c:10]1[CH2:11][NH:12][CH:13]1[CH2:14][CH2:15][N:16]([CH2:17][c:18]2[cH:19][cH:20][cH:21][cH:22][cH:23]2)[CH2:24][CH2:25]1>>[O:1]=[S:2]1(=[O:3])[NH:4][c:5]2[cH:6][cH:7][cH:8][cH:9][c:10]2[CH2:11][N:12]1[CH:13]1[CH2:14][CH2:15][N:16]([CH2:17][c:18]2[cH:19][cH:...
NS(N)(=O)=O.Nc1ccccc1CNC1CCN(Cc2ccccc2)CC1
O=S1(=O)Nc2ccccc2CN1C1CCN(Cc2ccccc2)CC1
null
null
N1=CC=CC=C1
Heteroatom Alkylation and Arylation
OtherReaction
b6b3b5cefac03fb1305f8cf424bdaa7abe03f5a0bb5812c3475110522a1d2b02
b397e30a6ccc587e05245a90512edc37f945dcc48b8cf6366dd21901a04fa1ba
O=S1(=O)Nc2ccccc2CN1C1CCN(Cc2ccccc2)CC1
N-[S;H0;D4;+0:1](-[NH2;D1;+0:2])(=[O;D1;H0:3])=[O;D1;H0:4].N-[c;H0;D3;+0:5](:[c:6]:[c:7]):[c:8](-[C:9]-[NH;D2;+0:10]-[C:11](-[C:12])-[C:13]):[c:14]>>[C:12]-[C:11](-[N;H0;D3;+0:10]1-[C:9]-[c:8](:[c:14]):[c;H0;D3;+0:5](:[c:6]:[c:7])-[NH;D2;+0:2]-[S;H0;D4;+0:1]-1(=[O;D1;H0:3])=[O;D1;H0:4])-[C:13]
null
[]
null
null
null
null
A solution of 11.0 g (0.0372 mol) of 2-amino-N-[1-(phenylmethyl)-4-piperidinyl]-benzenemethanamine in 200 ml of pyridine was added dropwise within 1.5 hours and at reflux temperature to a solution of 3.4 g (0.0354 mol) of sulphamide in 200 ml of pyridine and the mixture was then refluxed for 6 hours. The mixture was fr...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Sulfonamide.Primary amine.Secondary amine
Sulfonamide.Tertiary amine
c1ccccc1
c1ccc2c(c1)C[NH]SN2
c1ccc2c(c1)C[NH]SN2.C1CC[NH]CC1.c1ccccc1
Other
N1=CC=CC=C1
null
null
NS(N)(=O)=O.Nc1ccccc1CNC1CCN(Cc2ccccc2)CC1>N1=CC=CC=C1>O=S1(=O)Nc2ccccc2CN1C1CCN(Cc2ccccc2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-926f7b0a23cc4338b77caa0fd2afa495
BrBr.CC(=O)Nc1ccccc1C(C)=O>>CC(=O)Nc1ccccc1C(=O)CBr
BrBr.C(C)(=O)NC1=C(C=CC=C1)C(C)=O>>C(C)(=O)NC1=C(C=CC=C1)C(CBr)=O
Br[Br:14].[CH3:1][C:2](=[O:3])[NH:4][c:5]1[cH:6][cH:7][cH:8][cH:9][c:10]1[C:11](=[O:12])[CH3:13]>>[CH3:1][C:2](=[O:3])[NH:4][c:5]1[cH:6][cH:7][cH:8][cH:9][c:10]1[C:11](=[O:12])[CH2:13][Br:14]
BrBr.CC(=O)Nc1ccccc1C(C)=O
CC(=O)Nc1ccccc1C(=O)CBr
null
null
C(Cl)(Cl)Cl
Functional Group Interconversion
Bromination
97ca6720945af5a02c450d33ec56e946521050f9771c27f9cfcb85f3477593f6
cb3e14519230141aa015a4cf9c960def3e60f01997e61621f62506924bfa15de
c1ccccc1
Br-[Br;H0;D1;+0:1].[CH3;D1;+0:2]-[C:3](=[O;D1;H0:4])-[c:5]>>[Br;H0;D1;+0:1]-[CH2;D2;+0:2]-[C:3](=[O;D1;H0:4])-[c:5]
null
[]
null
null
null
null
45.0 g (0.282 mol) of dry bromine were added dropwise to a boiling solution of 50.0 g (0.282 mol) of 1-[2-(acetylamino)phenyl]ethanone in 400 ml of chloroform at room temperature. The solvent was distilled off, the residue was distributed between dichloromethane and saturated ice-cold sodium hydrogen carbonate solution...
10.6084/m9.figshare.5104873.v1
null
Ketone
Primary halide
null
null
c1ccccc1
HBr
C(Cl)(Cl)Cl
null
null
BrBr.CC(=O)Nc1ccccc1C(C)=O>C(Cl)(Cl)Cl>CC(=O)Nc1ccccc1C(=O)CBr
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0c9ef28bfebc44cb821975586637595e
CC(=O)Nc1ccccc1C(=O)CBr.CCN(C(C)C)C(C)C.N#C[O-].NC1CCN(Cc2ccccc2)CC1>>CC(=O)Nc1ccccc1-c1cccc2c1[nH]c(=O)n2C1CCN(Cc2ccccc2)CC1
NC1CCN(CC1)CC1=CC=CC=C1.CCN(C(C)C)C(C)C.C(C)(=O)NC1=C(C=CC=C1)C(CBr)=O.ClCCl.ClCCl.[O-]C#N.[Na+]>>C(C)(=O)NC1=C(C=CC=C1)C1=CC=CC=2N(C(NC21)=O)C2CCN(CC2)CC2=CC=CC=C2
O=[C:11]([c:10]1[c:5]([NH:4][C:2]([CH3:1])=[O:3])[cH:6][cH:7][cH:8][cH:9]1)[CH2:16]Br.CC(C)N([CH2:14][CH3:13])[CH:15](C)C.[N:17]#[C:18][O-:19].[NH2:20][CH:21]1[CH2:22][CH2:23][N:24]([CH2:25][c:26]2[cH:27][cH:28][cH:29][cH:30][cH:31]2)[CH2:32][CH2:33]1>>[CH3:1][C:2](=[O:3])[NH:4][c:5]1[cH:6][cH:7][cH:8][cH:9][c:10]1-[c:...
CC(=O)Nc1ccccc1C(=O)CBr.CCN(C(C)C)C(C)C.N#C[O-].NC1CCN(Cc2ccccc2)CC1
CC(=O)Nc1ccccc1-c1cccc2c1[nH]c(=O)n2C1CCN(Cc2ccccc2)CC1
null
null
C(C)(=O)OCC.CO.C(C)(=O)O
Aromatic Heterocycle Formation
OtherReaction
22e0571356f9b4546f1a6f12dd95cfce26ead01636f86f17c3d07e188843b96c
19b234a2c18b40db1eaf3feabf89dba2808f77a81cb843547290f6bdf88c8551
O=c1[nH]c2c(-c3ccccc3)cccc2n1C1CCN(Cc2ccccc2)CC1
Br-[CH2;D2;+0:1]-[C;H0;D3;+0:2](=O)-[c;H0;D3;+0:3](:[c:4]:[c:5]):[c:6](-[#7:7]-[C:8](-[C;D1;H3:9])=[O;D1;H0:10]):[c:11].C-C(-C)-N(-[CH2;D2;+0:12]-[CH3;D1;+0:13])-[CH;D3;+0:14](-C)-C.[C:15]-[C:16](-[NH2;D1;+0:17])-[C:18].[N;H0;D1;+0:19]#[C;H0;D2;+0:20]-[O-;H0;D1:21]>>[C:15]-[C:16](-[n;H0;D3;+0:17]1:[c;H0;D3;+0:14]2:[cH;...
null
[]
null
null
2
HOUR
To a solution of 26.3 g (0.138 mol) of 4-amino-1-(phenylmethyl)piperidine and 17.8 g (0.138 mol) of DIEA in 300 ml of dichloromethane was added dropwise a solution of 35.4 g (0.138 mol) of 1-[2-(acetylamino)phenyl]-2-bromoethanone in 150 ml of dichloromethane and the mixture was kept for a further 2 hours at room tempe...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ketone.Nitrile.Primary amine.Tertiary amine
null
null
c1ccc2[nH]cnc2c1
c1ccccc1.c1ccc2[nH]cnc2c1.C1CC[NH]CC1.c1ccccc1
HBr
C(C)(=O)OCC.CO.C(C)(=O)O
null
2
CC(=O)Nc1ccccc1C(=O)CBr.CCN(C(C)C)C(C)C.N#C[O-].NC1CCN(Cc2ccccc2)CC1>C(C)(=O)OCC.CO.C(C)(=O)O>CC(=O)Nc1ccccc1-c1cccc2c1[nH]c(=O)n2C1CCN(Cc2ccccc2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9bded59d75a645acb5b742b039b9008e
CC(=O)Nc1ccccc1-c1cn(C2CCN(Cc3ccccc3)CC2)c(=O)[nH]1>>Nc1ccccc1-c1cn(C2CCN(Cc3ccccc3)CC2)c(=O)[nH]1
C(C)(=O)NC1=C(C=CC=C1)C=1NC(N(C1)C1CCN(CC1)CC1=CC=CC=C1)=O.[OH-].[Na+]>>NC1=C(C=CC=C1)C=1NC(N(C1)C1CCN(CC1)CC1=CC=CC=C1)=O
CC(=O)[NH:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1-[c:8]1[cH:9][n:10]([CH:11]2[CH2:12][CH2:13][N:14]([CH2:15][c:16]3[cH:17][cH:18][cH:19][cH:20][cH:21]3)[CH2:22][CH2:23]2)[c:24](=[O:25])[nH:26]1>>[NH2:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1-[c:8]1[cH:9][n:10]([CH:11]2[CH2:12][CH2:13][N:14]([CH2:15][c:16]3[cH:17][cH:18][cH...
CC(=O)Nc1ccccc1-c1cn(C2CCN(Cc3ccccc3)CC2)c(=O)[nH]1
Nc1ccccc1-c1cn(C2CCN(Cc3ccccc3)CC2)c(=O)[nH]1
null
null
C(C)O
Reduction
Hydrogenolysis of amides/imides/carbamates
755df58c254dea764fdda078ffd678ec540bba057c83683be04c253f1270ac7b
025f7cefe51e71668ad5d09fca32df168e9b538347403e4d5c1748073e538adc
O=c1[nH]c(-c2ccccc2)cn1C1CCN(Cc2ccccc2)CC1
C-C(=O)-[NH;D2;+0:1]-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
A mixture of 3.0 g (7.68 mmol) of 4-[2-(acetylamino)phenyl]-1,3-dihydro-1-[1-(phenylmethyl)-4-piperidinyl]-2H-imidazol-2-one, 50 ml of 5 N sodium hydroxide solution and 25 ml of ethanol was refluxed for 3 hours. After cooling the organic phase was separated off, dried over sodium sulphate and evaporated down in vacuo. ...
10.6084/m9.figshare.5104873.v1
null
Secondary amide
Primary amine
null
null
c1ccccc1.c1c[nH]cn1.C1CC[NH]CC1.c1ccccc1
HO-
C(C)O
null
null
CC(=O)Nc1ccccc1-c1cn(C2CCN(Cc3ccccc3)CC2)c(=O)[nH]1>C(C)O>Nc1ccccc1-c1cn(C2CCN(Cc3ccccc3)CC2)c(=O)[nH]1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-24ab265129514a1faacd700f780a30a3
C=O.Nc1ccccc1-c1cn(C2CCN(Cc3ccccc3)CC2)c(=O)[nH]1>>O=c1[nH]c2c3ccccc3ncc2n1C1CCN(Cc2ccccc2)CC1
NC1=C(C=CC=C1)C=1NC(N(C1)C1CCN(CC1)CC1=CC=CC=C1)=O.C=O>>C1(=CC=CC=C1)CN1CCC(CC1)N1C(NC2=C1C=NC=1C=CC=CC21)=O
O=[CH2:12].[O:1]=[c:2]1[nH:3][c:4](-[c:5]2[cH:6][cH:7][cH:8][cH:9][c:10]2[NH2:11])[cH:13][n:14]1[CH:15]1[CH2:16][CH2:17][N:18]([CH2:19][c:20]2[cH:21][cH:22][cH:23][cH:24][cH:25]2)[CH2:26][CH2:27]1>>[O:1]=[c:2]1[nH:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][cH:9][c:10]3[n:11][cH:12][c:13]2[n:14]1[CH:15]1[CH2:16][CH2:17][N:18]([CH...
C=O.Nc1ccccc1-c1cn(C2CCN(Cc3ccccc3)CC2)c(=O)[nH]1
O=c1[nH]c2c3ccccc3ncc2n1C1CCN(Cc2ccccc2)CC1
null
null
C(Cl)(Cl)Cl
Aromatic Heterocycle Formation
OtherReaction
1b4fbe9ba18bc2d6b0b4c110dc5aeab38259cba7aa06bf91653c1dbde5322e8c
2f683162edeeaf0c6befa932010538b477a0290a1dac1031381b95d746c912ec
O=c1[nH]c2c3ccccc3ncc2n1C1CCN(Cc2ccccc2)CC1
O=[CH2;D1;+0:1].[C:2]-[#7;a:3]1:[cH;D2;+0:4]:[c;H0;D3;+0:5](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9](-[NH2;D1;+0:10]):[c:11]):[#7;a:12]:[c:13]:1=[O;D1;H0:14]>>[C:2]-[#7;a:3]1:[c:13](=[O;D1;H0:14]):[#7;a:12]:[c;H0;D3;+0:5]2:[c;H0;D3;+0:4]:1:[cH;D2;+0:1]:[n;H0;D2;+0:10]:[c:9](:[c:11]):[c;H0;D3;+0:6]:2:[c:7]:[c:8]
null
[]
null
null
1
HOUR
A solution of 2.67 g (7.66 mmol) of 4-(2-aminophenyl)-1,3-dihydro-1-[1-(phenylmethyl)-4-piperidinyl]-2H-imidazol-2-one in 50 ml of chloroform was mixed with 3.0 g of paraformaldehyde and refluxed for 3.5 hours. The residue remaining after evaporation of the solvent was taken up in 100 ml of methanol and acidified with ...
10.6084/m9.figshare.5104873.v1
null
Formaldehyde.Primary amine
null
c1c[nH]cn1.c1ccccc1
c1ccc2c(c1)ncc1nc[nH]c12
c1ccc2c(c1)ncc1nc[nH]c12.C1CC[NH]CC1.c1ccccc1
HO-
C(Cl)(Cl)Cl
null
1
C=O.Nc1ccccc1-c1cn(C2CCN(Cc3ccccc3)CC2)c(=O)[nH]1>C(Cl)(Cl)Cl>O=c1[nH]c2c3ccccc3ncc2n1C1CCN(Cc2ccccc2)CC1