dataset_id
large_stringclasses
414 values
reaction_id
large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
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large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-573e8af24c15454793a5a9bb824c9cdf
Brc1cnc(Nc2ccc(OCCN3CCOCC3)cc2)c2ncnn12.CC1(C)OB(c2csc(C(N)=O)c2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1>>N.NC(=O)c1cc(-c2cnc(Nc3ccc(OCCN4CCOCC4)cc3)c3ncnn23)cs1
CC1(OB(OC1(C)C)C=1C=C(SC1)C(=O)N)C.CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2.C(=O)([O-])[O-].[Na+].[Na+].BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)OCCN2CCOCC2>>N.O1CCN(CC1)CCOC1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2
Br[c:8]1[cH:9][n:10][c:11]([NH:12][c:13]2[cH:14][cH:15][c:16]([O:17][CH2:18][CH2:19][N:20]3[CH2:21][CH2:22][O:23][CH2:24][CH2:25]3)[cH:26][cH:27]2)[c:28]2[n:29][cH:30][n:31][n:32]12.CC1(C)OB(c2csc(C(=O)[NH2:1])c2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-[c:7]4[cH:6][c:5]([C:3]([NH2:2])=[O:4])[s:34][cH:33]4)n4ncnc34)cc2)CC1>>[NH3:1...
Brc1cnc(Nc2ccc(OCCN3CCOCC3)cc2)c2ncnn12.CC1(C)OB(c2csc(C(N)=O)c2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1
N.NC(=O)c1cc(-c2cnc(Nc3ccc(OCCN4CCOCC4)cc3)c3ncnn23)cs1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O1CCOCC1
C-C Coupling
OtherReaction
5d4ca946d437df36dd96fd1b6d9c8cdde8fc4524e5bae3cb1f7cc44766204f15
96e5f3628c1bd4659dd3e9821904115decf673d0e8e42bb7900b7f521b084c51
c1nc2c(Nc3ccc(OCCN4CCOCC4)cc3)ncc(-c3ccsc3)n2n1
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1.C-C1(-C)-O-B(-c2:c:s:c(-C(=O)-[NH2;D1;+0:10]):c:2)-O-C-1(-C)-C.C-N1-C-C-N(-c2:c:c:c(-N-c3:n:c:c(-[c;H0;D3;+0:11]4:[c:12]:[#16;a:13]:[c:14](-[C:15](-[N;D1;H2:16])=[O;D1;H0:17]):[c:18]:4):n4:n:c:n:c:3:4):c:c:2)-C-C-1>>[N;D1;H2:16]-[C:15](...
52
[{"value": 52.0, "product": "O1CCN(CC1)CCOC1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound may be prepared using methods as described for Compound 6, step 4, using (5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-yl)-[4-(2-morpholin-4-yl-ethoxy)-phenyl]-amine (113 mg, 0.27 mmol), 4-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-thiophene-2-carboxamide (136 mg, 0.537 mmol), and Pd(PPh3)4 (78 mg, 0.067 m...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amide.Secondary amine.Tertiary amine.Tertiary amine.Boronic ester
null
c1cn2ncnc2cn1.B1OCCO1.c1ccsc1.C1CNCCN1.c1ccccc1.c1ccsc1.c1cn2ncnc2cn1
c1ccsc1.c1cn2ncnc2cn1
c1ccsc1.c1ccccc1.C1COCC[NH]1.c1cn2ncnc2cn1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1
null
null
Brc1cnc(Nc2ccc(OCCN3CCOCC3)cc2)c2ncnn12.CC1(C)OB(c2csc(C(N)=O)c2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1>N.NC(=O)c1cc(...
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a9c6a97dd90f40e88c5dd30e4580df9e
Brc1cnc(Nc2ccc(OCCN3CCOCC3)cc2)c2ncnn12.CC1(C)OB(c2ccc(C(N)=O)s2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1>>N.NC(=O)c1ccc(-c2cnc(Nc3ccc(OCCN4CCOCC4)cc3)c3ncnn23)s1
CC1(OB(OC1(C)C)C1=CC=C(S1)C(=O)N)C.CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2.C(=O)([O-])[O-].[Na+].[Na+].BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)OCCN2CCOCC2>>N.O1CCN(CC1)CCOC1=CC=C(C=C1)NC=1C=2N(C(=CN1)C1=CC=C(S1)C(=O)N)N=CN2
Br[c:9]1[cH:10][n:11][c:12]([NH:13][c:14]2[cH:15][cH:16][c:17]([O:18][CH2:19][CH2:20][N:21]3[CH2:22][CH2:23][O:24][CH2:25][CH2:26]3)[cH:27][cH:28]2)[c:29]2[n:30][cH:31][n:32][n:33]12.CC1(C)OB([c:8]2[cH:7][cH:6][c:5]([C:3]([NH2:2])=[O:4])[s:34]2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(=O)[NH2:1])c4)n4ncnc34)cc2)CC1>>[NH3:1...
Brc1cnc(Nc2ccc(OCCN3CCOCC3)cc2)c2ncnn12.CC1(C)OB(c2ccc(C(N)=O)s2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1
N.NC(=O)c1ccc(-c2cnc(Nc3ccc(OCCN4CCOCC4)cc3)c3ncnn23)s1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O1CCOCC1
C-C Coupling
OtherReaction
5d4ca946d437df36dd96fd1b6d9c8cdde8fc4524e5bae3cb1f7cc44766204f15
96e5f3628c1bd4659dd3e9821904115decf673d0e8e42bb7900b7f521b084c51
c1csc(-c2cnc(Nc3ccc(OCCN4CCOCC4)cc3)c3ncnn23)c1
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1.C-C1(-C)-O-B(-[c;H0;D3;+0:10]2:[#16;a:11]:[c:12](-[C:13](-[N;D1;H2:14])=[O;D1;H0:15]):[c:16]:[c:17]:2)-O-C-1(-C)-C.C-N1-C-C-N(-c2:c:c:c(-N-c3:n:c:c(-c4:c:s:c(-C(=O)-[NH2;D1;+0:18]):c:4):n4:n:c:n:c:3:4):c:c:2)-C-C-1>>[N;D1;H2:14]-[C:13](...
25
[{"value": 25.0, "product": "O1CCN(CC1)CCOC1=CC=C(C=C1)NC=1C=2N(C(=CN1)C1=CC=C(S1)C(=O)N)N=CN2", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound may be prepared using methods as described for Compound 6, step 4, using (5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-yl)-[4-(2-morpholin-4-yl-ethoxy)-phenyl]-amine (118 mg, 0.28 mmol), 5-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-thiophene-2-carboxamide (142 mg, 0.56 mmol), and Pd(PPh3)4 (81 mg, 0.07 mmo...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amide.Secondary amine.Tertiary amine.Tertiary amine.Boronic ester
null
c1cn2ncnc2cn1.B1OCCO1.c1ccsc1.C1CNCCN1.c1ccccc1.c1ccsc1.c1cn2ncnc2cn1
c1ccsc1.c1cn2ncnc2cn1
c1ccsc1.c1ccccc1.C1COCC[NH]1.c1cn2ncnc2cn1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1
null
null
Brc1cnc(Nc2ccc(OCCN3CCOCC3)cc2)c2ncnn12.CC1(C)OB(c2ccc(C(N)=O)s2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1>N.NC(=O)c1ccc...
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8f528335182e4588bf47d51a6b6245a2
C1=COCCC1.c1cn[nH]c1>>c1cnn(C2CCCCO2)c1
N1N=CC=C1.O1CCCC=C1>>O1C(CCCC1)N1N=CC=C1
[CH:5]1=[CH:6][CH2:7][CH2:8][CH2:9][O:10]1.[cH:1]1[cH:2][n:3][nH:4][cH:11]1>>[cH:1]1[cH:2][n:3][n:4]([CH:5]2[CH2:6][CH2:7][CH2:8][CH2:9][O:10]2)[cH:11]1
C1=COCCC1.c1cn[nH]c1
c1cnn(C2CCCCO2)c1
null
[H-].[Na+].C(=O)(C(F)(F)F)O
null
Heteroatom Alkylation and Arylation
OtherReaction
1ec778c8f54d7ad18e95009f54038d9cdb57b9e363777849f1433a4ce7a5e2cb
c37c4c64b8e0c6e5b39694c16f8c97245b55f05530ce8b5df4dfb3a695b50244
c1cnn(C2CCCCO2)c1
[#7;a:1]1:[c:2]:[c:3]:[c:4]:[nH;D2;+0:5]:1.[#8:6]1-[C:7]-[C:8]-[C:9]-[CH;D2;+0:10]=[CH;D2;+0:11]-1>>[#7;a:1]1:[c:2]:[c:3]:[c:4]:[n;H0;D3;+0:5]:1-[CH;D3;+0:11]1-[#8:6]-[C:7]-[C:8]-[C:9]-[CH2;D2;+0:10]-1
104.2
[{"value": 99.0, "product": "O1C(CCCC1)N1N=CC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 104.2, "product": "O1C(CCCC1)N1N=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
95
CELSIUS
5
HOUR
1H-Pyrazole (14.3 g, 0.21 mol) is dissolved in 3,4-dihydro-2H-pyran (26.74 g, 0.32 mol) in the presence of a catalytic amount of TFA (0.1 mL, 1.3 mmol). The reaction mixture is stirred at 95° C. for 5 hours, cooled and then quenched using NaH (0.2 g, 5 mmol). The solvent is removed to give the title compound as a brown...
10.6084/m9.figshare.5104873.v1
null
Ether
Ether
C1=COCCC1.c1cn[nH]c1
c1cn[nH]c1.C1CCOCC1
c1cn[nH]c1.C1CCOCC1
null
[H-].[Na+].C(=O)(C(F)(F)F)O
95
5
C1=COCCC1.c1cn[nH]c1>[H-].[Na+].C(=O)(C(F)(F)F)O>c1cnn(C2CCCCO2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-033ea64afce44276a7c4dac91d4384c8
CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1.Nc1ccc(N2CCOCC2)cc1.OB(O)N1CC=CN1>>c1cc(-c2cnc(Nc3ccc(N4CCOCC4)cc3)c3ncnn23)[nH]n1
CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2.N1N(CC=C1)B(O)O.C(=O)([O-])[O-].[Na+].[Na+].N1(CCOCC1)C1=CC=C(C=C1)N>>N1(CCOCC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1NN=CC1)N=CN2
CN1CCN(c2cc[c:9]([NH:8][c:7]3[n:6][cH:5][c:4](-[c:3]4cs[c:1](C(N)=O)[cH:2]4)[n:25]4[c:21]3[n:22][cH:23][n:24]4)[cH:20]c2)CC1.Nc1c[cH:19][c:12]([N:13]2[CH2:14][CH2:15][O:16][CH2:17][CH2:18]2)[cH:11][cH:10]1.OB(O)[N:26]1CC=C[NH:27]1>>[cH:1]1[cH:2][c:3](-[c:4]2[cH:5][n:6][c:7]([NH:8][c:9]3[cH:10][cH:11][c:12]([N:13]4[CH2:...
CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1.Nc1ccc(N2CCOCC2)cc1.OB(O)N1CC=CN1
c1cc(-c2cnc(Nc3ccc(N4CCOCC4)cc3)c3ncnn23)[nH]n1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
CN(C)C=O.C(=O)(O)[O-].[Na+]
Miscellaneous
OtherReaction
382fe5a33715f095223f38950c48bec08e32887180f353c786d0a7db211a916e
76c182260d9c73fd569006c43f3814f68c8d83080194fb7784bbe2c269a8e6b9
c1cc(-c2cnc(Nc3ccc(N4CCOCC4)cc3)c3ncnn23)[nH]n1
C-N1-C-C-N(-c2:c:[cH;D2;+0:1]:[c;H0;D3;+0:2](-[#7:3]-[c:4]3:[#7;a:5]:[c:6]:[c:7](-[c;H0;D3;+0:8]4:[c:9]:[c;H0;D3;+0:10](-C(-N)=O):s:c:4):[#7;a:11]4:[#7;a:12]:[c:13]:[#7;a:14]:[c:15]:4:3):c:c:2)-C-C-1.N-c1:[cH;D2;+0:16]:[c:17]:[c:18](-[#7:19]):[cH;D2;+0:20]:c:1.O-B(-O)-[N;H0;D3;+0:21]1-C-C=C-[NH;D2;+0:22]-1>>[#7:19]-[c:...
null
[]
100
CELSIUS
18
HOUR
This compound may be prepared using methods as described for Compound 6, step 4, using 5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-yl)-[4-(morpholin-4-yl)-phenyl]-amine (100 mg, 0.267 mmol), 1H-pyrazole-2-boronic acid (60 mg, 0.535 mmol), Pd(PPh3)4 (93 mg, 0.08 mmol) and Na2CO3 (88 mg, 0.80 mmol) in DMF (2 mL). The reactio...
10.6084/m9.figshare.5104873.v1
null
Enamine.Hydrazine.Primary amide.Primary amine.Tertiary amine.Tertiary amine
null
C1CNCCN1.c1ccccc1.c1ccsc1.c1ccccc1.C1=CN[NH]C1
c1cn[nH]c1.c1ccccc1
c1cn[nH]c1.c1ccccc1.C1COCC[NH]1.c1cn2ncnc2cn1
B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.CN(C)C=O.C(=O)(O)[O-].[Na+]
100
18
CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1.Nc1ccc(N2CCOCC2)cc1.OB(O)N1CC=CN1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.CN(C)C=O.C(=O)(O)[O-].[Na+]>c1cc(-c2cnc(Nc3ccc(N4CCOCC4)cc3)c...
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e19017422ab14010904dfe523c48205d
CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cn2)CC1.CC1(C)OB(c2csc(C(N)=O)c2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1>>CC(C)N1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1.N
CC1(OB(OC1(C)C)C=1C=C(SC1)C(=O)N)C.CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2.C(=O)([O-])[O-].[Na+].[Na+].BrC1=CN=C(C=2N1N=CN2)NC=2C=NC(=CC2)N2CCN(CC2)C(C)C>>N.C(C)(C)N1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2
Br[c:16]1[cH:15][n:14][c:13]([NH:12][c:11]2[cH:10][cH:9][c:8]([N:7]3[CH2:6][CH2:5][N:4]([CH:2]([CH3:1])[CH3:3])[CH2:33][CH2:32]3)n[cH:30]2)[c:29]2[n:25]1[n:26][cH:27][n:28]2.CC1(C)OB([c:17]2[cH:18][s:19][c:20]([C:21]([NH2:22])=[O:23])[cH:24]2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(=O)[NH2:34])c4)n4ncnc34)c[cH:31]2)CC1>>[...
CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cn2)CC1.CC1(C)OB(c2csc(C(N)=O)c2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1
CC(C)N1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1.N
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O1CCOCC1
C-C Coupling
OtherReaction
cf5549799cc4acd18ed81259f1840ced3dc52c62c8411c2248454740f4743d6e
96e5f3628c1bd4659dd3e9821904115decf673d0e8e42bb7900b7f521b084c51
c1nc2c(Nc3ccc(N4CCNCC4)cc3)ncc(-c3ccsc3)n2n1
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4](-[#7:5]-[c:6]2:[c:7]:[c:8]:[c;H0;D3;+0:9](-[#7:10](-[C:11])-[C:12]):n:[cH;D2;+0:13]:2):[c:14]2:[#7;a:15]:[c:16]:[#7;a:17]:[#7;a:18]:2:1.C-C1(-C)-O-B(-[c;H0;D3;+0:19]2:[c:20]:[#16;a:21]:[c:22](-[C:23](-[N;D1;H2:24])=[O;D1;H0:25]):[c:26]:2)-O-C-1(-C)-C.C-N1-C-C-N(-c2:[cH;D2;+0:27]:...
61
[{"value": 61.0, "product": "C(C)(C)N1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound may be prepared using methods as described for Compound 6, step 4, using 5-bromo-N-(6-(4-isopropylpiperazin-1-yl)pyridin-3-yl)-[1,2,4]triazolo[1,5-a]pyrazin-8-amine (100 mg, 0.24 mmol), 4-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-thiophene-2-carboxamide (121 mg, 0.48 mmol), and Pd(PPh3)4 (69 mg, 0.05...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amide.Secondary amine.Tertiary amine.Tertiary amine.Boronic ester
null
c1ccncc1.c1cn2ncnc2cn1.B1OCCO1.c1ccsc1.C1CNCCN1.c1ccccc1.c1ccsc1.c1cn2ncnc2cn1
c1ccccc1.c1ccsc1.c1cn2ncnc2cn1
C1C[NH]CC[NH]1.c1ccccc1.c1ccsc1.c1cn2ncnc2cn1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1
null
null
CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cn2)CC1.CC1(C)OB(c2csc(C(N)=O)c2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1>CC(C)N1CC...
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4682667b785a4aff8b0f28ad39cf080c
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1cnc(N(C(=O)OC(C)(C)C)c2ccc(N3CCOCC3)cc2)c2ncnn12.NC(=O)c1coc(Br)c1>>CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1)c1ncc(-c2cc(C(N)=O)co2)n2ncnc12.N
BrC1=CC(=CO1)C(=O)N.C(C)(C)(C)OC(N(C=1C=2N(C(=CN1)[Sn](CCCC)(CCCC)CCCC)N=CN2)C2=CC=C(C=C2)N2CCOCC2)=O>>N.C(C)(C)(C)OC(N(C1=CC=C(C=C1)N1CCOCC1)C=1C=2N(C(=CN1)C=1OC=C(C1)C(N)=O)N=CN2)=O
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c:24]1[cH:23][n:22][c:21]([N:8]([C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[c:9]2[cH:10][cH:11][c:12]([N:13]3[CH2:14][CH2:15][O:16][CH2:17][CH2:18]3)[cH:19][cH:20]2)[c:37]2[n:33]1[n:34][cH:35][n:36]2.Br[c:25]1[cH:26][c:27]([C:28]([NH2:29])=[O:30])[cH:31][o:32]1>>[CH3:1][C:2]([CH3:...
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1cnc(N(C(=O)OC(C)(C)C)c2ccc(N3CCOCC3)cc2)c2ncnn12.NC(=O)c1coc(Br)c1
CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1)c1ncc(-c2cc(C(N)=O)co2)n2ncnc12.N
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
CN(C)C=O
C-C Coupling
Stille reaction_aryl
2d93a19b76dcf287bebe9ba413007f5f606bbf0e5afcd12afd99e2d0ec809644
db27eeefac0475c6d74fa10b3167e95a61caaae74e8bbafd45892452c0c3d4d6
c1coc(-c2cnc(Nc3ccc(N4CCOCC4)cc3)c3ncnn23)c1
Br-[c;H0;D3;+0:1]1:[#8;a:2]:[c:3]:[c:4](-[C:5](-[N;D1;H2:6])=[O;D1;H0:7]):[c:8]:1.C-C-C-[CH2]-[Sn](-[CH2]-C-C-C)(-[CH2]-C-C-C)-[c;H0;D3;+0:9]1:[c:10]:[#7;a:11]:[c:12]:[c:13]2:[#7;a:14]:[c:15]:[#7;a:16]:[#7;a:17]:2:1>>[N;D1;H2:6]-[C:5](=[O;D1;H0:7])-[c:4]1:[c:8]:[c;H0;D3;+0:1](-[c;H0;D3;+0:9]2:[c:10]:[#7;a:11]:[c:12]:[c...
65.6
[{"value": 33.0, "product": "C(C)(C)(C)OC(N(C1=CC=C(C=C1)N1CCOCC1)C=1C=2N(C(=CN1)C=1OC=C(C1)C(N)=O)N=CN2)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 65.6, "product": "C(C)(C)(C)OC(N(C1=CC=C(C=C1)N1CCOCC1)C=1C=2N(C(=CN1)C=1OC=C(C1)C(N)=O)N=CN2)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": f...
null
null
null
null
This compound may be prepared using methods as described for Compound 35, step 3 using (4-morpholin-4-yl-phenyl)-(5-tributylstannanyl-[1,2,4]triazolo[1,5-a]pyrazin-8-yl)-carbamic acid tert-butyl ester (137 mg, 0.199 mmol), 5-bromo-furan-3-carboxamide (76 mg, 0.4 mmol) and Pd(PPh3)4 (23 mg, 0.020 mmol) in DMF (1 mL). Pu...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Tin
null
c1cn2ncnc2cn1.c1ccoc1
c1ccoc1.c1cn2ncnc2cn1
c1ccccc1.C1COCC[NH]1.c1ccoc1.c1cn2ncnc2cn1
HBr.Sn
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.CN(C)C=O
null
null
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1cnc(N(C(=O)OC(C)(C)C)c2ccc(N3CCOCC3)cc2)c2ncnn12.NC(=O)c1coc(Br)c1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.CN(C)C=O>CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1)c1...
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b9266df4202d4b82be65878f09012599
CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1)c1ncc(-c2cc(C(N)=O)co2)n2ncnc12>>NC(=O)c1coc(-c2cnc(Nc3ccc(N4CCOCC4)cc3)c3ncnn23)c1
C(C)(C)(C)OC(N(C1=CC=C(C=C1)N1CCOCC1)C=1C=2N(C(=CN1)C=1OC=C(C1)C(N)=O)N=CN2)=O.C(=O)([O-])[O-].[Na+].[Na+]>>O1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C1=CC(=CO1)C(=O)N)N=CN2
CC(C)(C)OC(=O)[N:12]([c:11]1[n:10][cH:9][c:8](-[c:7]2[o:6][cH:5][c:4]([C:2]([NH2:1])=[O:3])[cH:30]2)[n:29]2[c:25]1[n:26][cH:27][n:28]2)[c:13]1[cH:14][cH:15][c:16]([N:17]2[CH2:18][CH2:19][O:20][CH2:21][CH2:22]2)[cH:23][cH:24]1>>[NH2:1][C:2](=[O:3])[c:4]1[cH:5][o:6][c:7](-[c:8]2[cH:9][n:10][c:11]([NH:12][c:13]3[cH:14][cH...
CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1)c1ncc(-c2cc(C(N)=O)co2)n2ncnc12
NC(=O)c1coc(-c2cnc(Nc3ccc(N4CCOCC4)cc3)c3ncnn23)c1
null
C(=O)(C(F)(F)F)O
C(Cl)Cl
Reduction
Boc amine deprotection
bbda4640db5f48af4538caded12fdadd56eacd6d4e5f7aefe46282d665df167e
a94b29c7264c852156fc1cdd4a0951a4fc26c06d0edc9e50c743825dbf79e3fd
c1coc(-c2cnc(Nc3ccc(N4CCOCC4)cc3)c3ncnn23)c1
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1](-[c:2]1:[#7;a:3]:[c:4]:[c:5]:[#7;a:6]2:[#7;a:7]:[c:8]:[#7;a:9]:[c:10]:2:1)-[c:11](:[c:12]):[c:13]>>[c:12]:[c:11](-[NH;D2;+0:1]-[c:2]1:[#7;a:3]:[c:4]:[c:5]:[#7;a:6]2:[#7;a:7]:[c:8]:[#7;a:9]:[c:10]:2:1):[c:13]
null
[]
null
null
null
null
A solution of [5-(4-carbamoyl-furan-2-yl)-[1,2,4]triazolo[1,5-a]pyrazin-8-yl]-(4-morpholin-4-yl-phenyl)-carbamic acid tert-butyl ester (33 mg, 0.065 mmol) in a mixture 1:1 DCM:TFA (2 mL) (2 drops of water) is stirred at room temperature for 2 hours. After addition of sat. Na2CO3, a precipitate is formed, collected by f...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Secondary amine
null
null
c1ccoc1.c1ccccc1.C1COCC[NH]1.c1cn2ncnc2cn1
HO-
C(=O)(C(F)(F)F)O.C(Cl)Cl
null
null
CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1)c1ncc(-c2cc(C(N)=O)co2)n2ncnc12>C(=O)(C(F)(F)F)O.C(Cl)Cl>NC(=O)c1coc(-c2cnc(Nc3ccc(N4CCOCC4)cc3)c3ncnn23)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e6d1cc21a2374b188d7985459089b206
Brc1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12.CC1(C)OB(c2ccc3c(c2)CNC3=O)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1>>N.O=C1NCc2cc(-c3cnc(Nc4ccc(N5CCOCC5)cc4)c4ncnn34)ccc21
CC1(OB(OC1(C)C)C=1C=C2CNC(C2=CC1)=O)C.BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2CCOCC2.CC1(OB(OC1(C)C)C=1C=C2CNC(C2=CC1)=O)C.CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2>>N.O1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C3CNC(C3=CC1)=O)N=CN2
Br[c:9]1[cH:10][n:11][c:12]([NH:13][c:14]2[cH:15][cH:16][c:17]([N:18]3[CH2:19][CH2:20][O:21][CH2:22][CH2:23]3)[cH:24][cH:25]2)[c:26]2[n:27][cH:28][n:29][n:30]12.CC1(C)OB([c:8]2[cH:7][c:6]3[c:33]([cH:32][cH:31]2)[C:3](=[O:2])[NH:4][CH2:5]3)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(=O)[NH2:1])c4)n4ncnc34)cc2)CC1>>[NH3:1].[O:2...
Brc1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12.CC1(C)OB(c2ccc3c(c2)CNC3=O)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1
N.O=C1NCc2cc(-c3cnc(Nc4ccc(N5CCOCC5)cc4)c4ncnn34)ccc21
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O1CCOCC1.C(=O)([O-])[O-].[Na+].[Na+]
C-C Coupling
OtherReaction
d96e7a493e1619b343e6902e2f3e9ceea3531a747b8fbd8e81a720c753a845f2
96e5f3628c1bd4659dd3e9821904115decf673d0e8e42bb7900b7f521b084c51
O=C1NCc2cc(-c3cnc(Nc4ccc(N5CCOCC5)cc4)c4ncnn34)ccc21
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1.C-C1(-C)-O-B(-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14])-O-C-1(-C)-C.C-N1-C-C-N(-c2:c:c:c(-N-c3:n:c:c(-c4:c:s:c(-C(=O)-[NH2;D1;+0:15]):c:4):n4:n:c:n:c:3:4):c:c:2)-C-C-1>>[NH3;D0;+0:15].[c:12]:[c:11]:[c;H0;D3;+0:10](-[c;H0;D3;+0:1]1:...
79
[{"value": 79.0, "product": "O1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C3CNC(C3=CC1)=O)N=CN2", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound may be prepared using methods as described for Compound 6, step 4 using (5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-yl)-(4-morpholin-4-yl-phenyl)-amine (1.0 g, 2.67 mmol), 5-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-2,3-dihydro-isoindol-1-one (see description for Compound 79) (1.03 g, 4.01 mmol) and Pd(...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amide.Secondary amine.Tertiary amine.Tertiary amine.Boronic ester
null
c1cn2ncnc2cn1.B1OCCO1.c1ccc2c(c1)CNC2.C1CNCCN1.c1ccccc1.c1ccsc1.c1cn2ncnc2cn1
c1ccc2c(c1)CNC2.c1cn2ncnc2cn1
c1ccc2c(c1)CNC2.c1ccccc1.C1COCC[NH]1.c1cn2ncnc2cn1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1.C(=O)([O-])[O-].[Na+].[Na+]
null
null
Brc1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12.CC1(C)OB(c2ccc3c(c2)CNC3=O)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1.C(=O)([O-])[O-...
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2462972170de4c979b2ad2ad40df4acf
Brc1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12.CC1(C)OB(c2coc(C(N)=O)c2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1>>N.NC(=O)c1cc(-c2cnc(Nc3ccc(N4CCOCC4)cc3)c3ncnn23)co1
CC1(OB(OC1(C)C)C=1C=C(OC1)C(=O)N)C.CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2.C(=O)([O-])[O-].[Na+].[Na+].BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2CCOCC2>>N.O1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(OC1)C(=O)N)N=CN2
Br[c:8]1[cH:9][n:10][c:11]([NH:12][c:13]2[cH:14][cH:15][c:16]([N:17]3[CH2:18][CH2:19][O:20][CH2:21][CH2:22]3)[cH:23][cH:24]2)[c:25]2[n:26][cH:27][n:28][n:29]12.CC1(C)OB([c:7]2[cH:6][c:5]([C:3]([NH2:2])=[O:4])[o:31][cH:30]2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(=O)[NH2:1])c4)n4ncnc34)cc2)CC1>>[NH3:1].[NH2:2][C:3](=[O:4])...
Brc1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12.CC1(C)OB(c2coc(C(N)=O)c2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1
N.NC(=O)c1cc(-c2cnc(Nc3ccc(N4CCOCC4)cc3)c3ncnn23)co1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O1CCOCC1
C-C Coupling
OtherReaction
5cb7909cd8a8fb68256336e464d1363240b5ce9f1a1aa9f9849dc58e4e9eb2b6
96e5f3628c1bd4659dd3e9821904115decf673d0e8e42bb7900b7f521b084c51
c1nc2c(Nc3ccc(N4CCOCC4)cc3)ncc(-c3ccoc3)n2n1
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1.C-C1(-C)-O-B(-[c;H0;D3;+0:10]2:[c:11]:[#8;a:12]:[c:13](-[C:14](-[N;D1;H2:15])=[O;D1;H0:16]):[c:17]:2)-O-C-1(-C)-C.C-N1-C-C-N(-c2:c:c:c(-N-c3:n:c:c(-c4:c:s:c(-C(=O)-[NH2;D1;+0:18]):c:4):n4:n:c:n:c:3:4):c:c:2)-C-C-1>>[N;D1;H2:15]-[C:14](=...
65
[{"value": 65.0, "product": "O1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(OC1)C(=O)N)N=CN2", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound may be prepared using methods as described for Compound 6, step 4, using (5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-yl)-(4-morpholin-4-yl-phenyl)-amine (78 mg, 0.16 mmol), 4-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-furan-2-carboxylic acid amide (100 mg, 0.34 mmol), and Pd(PPh3)4 (60 mg, 0.052 mmol) in...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amide.Secondary amine.Tertiary amine.Tertiary amine.Boronic ester
null
c1cn2ncnc2cn1.B1OCCO1.c1ccoc1.C1CNCCN1.c1ccccc1.c1ccsc1.c1cn2ncnc2cn1
c1ccoc1.c1cn2ncnc2cn1
c1ccoc1.c1ccccc1.C1COCC[NH]1.c1cn2ncnc2cn1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1
null
null
Brc1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12.CC1(C)OB(c2coc(C(N)=O)c2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1>N.NC(=O)c1cc(-c2...
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4dc67b9fd0074c14b6e5e61824caa6be
CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1)c1ncc(Br)n2ncnc12.CCC[CH2][Sn]([Cl])([CH2]CCC)[CH2]CCC>>CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1cnc(N(C(=O)OC(C)(C)C)c2ccc(N3CCOCC3)cc2)c2ncnn12
C(C)(C)(C)OC(N(C1=CC=C(C=C1)N1CCOCC1)C=1C=2N(C(=CN1)Br)N=CN2)=O.C(C)(C)[Mg]Cl.C(CCC)[Sn](CCCC)(CCCC)Cl>>C(C)(C)(C)OC(N(C=1C=2N(C(=CN1)[Sn](CCCC)(CCCC)CCCC)N=CN2)C2=CC=C(C=C2)N2CCOCC2)=O
Br[c:14]1[cH:15][n:16][c:17]([N:18]([C:19](=[O:20])[O:21][C:22]([CH3:23])([CH3:24])[CH3:25])[c:26]2[cH:27][cH:28][c:29]([N:30]3[CH2:31][CH2:32][O:33][CH2:34][CH2:35]3)[cH:36][cH:37]2)[c:38]2[n:39][cH:40][n:41][n:42]12.[Cl][Sn:5]([CH2:4][CH2:3][CH2:2][CH3:1])([CH2:6][CH2:7][CH2:8][CH3:9])[CH2:10][CH2:11][CH2:12][CH3:13]...
CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1)c1ncc(Br)n2ncnc12.CCC[CH2][Sn]([Cl])([CH2]CCC)[CH2]CCC
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1cnc(N(C(=O)OC(C)(C)C)c2ccc(N3CCOCC3)cc2)c2ncnn12
null
null
C1CCOC1
Functional Group Interconversion
OtherReaction
858564ed3656a34d5d3476ad96880ed87dc5473e1498305aa6913cc5a6520b94
d9bf9bd3fc00efb5d713d9ac7f168986c2c94f1f455d32bdc9901567c1014c76
c1cn2ncnc2c(Nc2ccc(N3CCOCC3)cc2)n1
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1.[C:10]-[C:11]-[Sn;H0;D4;+0:12](-[Cl])(-[C:13]-[C:14])-[C:15]-[C:16]>>[C:10]-[C:11]-[Sn;H0;D4;+0:12](-[C:13]-[C:14])(-[C:15]-[C:16])-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1
null
[]
null
null
5
MINUTE
To a cooled (−78° C.) solution of (5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-yl)-(4-morpholin-4-yl-phenyl)-carbamic acid tert-butyl ester (370 mg, 0.78 mmol) in THF (12 mL), are added 2M isopropylmagnesium chloride in THF (0.78 mL, 1.56 mmol), and after 5 minutes stirring, tributyltin chloride (0.42, 1.56 mmol) is added....
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Tin
Tin
c1cn2ncnc2cn1
c1cn2ncnc2cn1
c1ccccc1.C1COCC[NH]1.c1cn2ncnc2cn1
Br-
C1CCOC1
null
0.083333
CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1)c1ncc(Br)n2ncnc12.CCC[CH2][Sn]([Cl])([CH2]CCC)[CH2]CCC>C1CCOC1>CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1cnc(N(C(=O)OC(C)(C)C)c2ccc(N3CCOCC3)cc2)c2ncnn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-67395b4e30f3477f8a384fb661774435
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1cnc(N(C(=O)OC(C)(C)C)c2ccc(N3CCOCC3)cc2)c2ncnn12.O=C1NCCc2cc(Br)ccc21>>CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1)c1ncc(-c2ccc3c(c2)CCNC3=O)n2ncnc12
C(C)(C)(C)OC(N(C=1C=2N(C(=CN1)[Sn](CCCC)(CCCC)CCCC)N=CN2)C2=CC=C(C=C2)N2CCOCC2)=O.BrC=1C=C2CCNC(C2=CC1)=O>>C(C)(C)(C)OC(N(C=1C=2N(C(=CN1)C=1C=C3CCNC(C3=CC1)=O)N=CN2)C2=CC=C(C=C2)N2CCOCC2)=O
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c:24]1[cH:23][n:22][c:21]([N:8]([C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[c:9]2[cH:10][cH:11][c:12]([N:13]3[CH2:14][CH2:15][O:16][CH2:17][CH2:18]3)[cH:19][cH:20]2)[c:40]2[n:36]1[n:37][cH:38][n:39]2.Br[c:25]1[cH:26][cH:27][c:28]2[c:29]([cH:30]1)[CH2:31][CH2:32][NH:33][C:34]2=[O:3...
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1cnc(N(C(=O)OC(C)(C)C)c2ccc(N3CCOCC3)cc2)c2ncnn12.O=C1NCCc2cc(Br)ccc21
CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1)c1ncc(-c2ccc3c(c2)CCNC3=O)n2ncnc12
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
CN(C)C=O
C-C Coupling
Stille reaction_aryl
aec2e584c41d2913f710da02512f5af7edead4672b622f92cfa7bacdc4552ce1
db27eeefac0475c6d74fa10b3167e95a61caaae74e8bbafd45892452c0c3d4d6
O=C1NCCc2cc(-c3cnc(Nc4ccc(N5CCOCC5)cc4)c4ncnn34)ccc21
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].C-C-C-[CH2]-[Sn](-[CH2]-C-C-C)(-[CH2]-C-C-C)-[c;H0;D3;+0:6]1:[c:7]:[#7;a:8]:[c:9]:[c:10]2:[#7;a:11]:[c:12]:[#7;a:13]:[#7;a:14]:2:1>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6]1:[c:7]:[#7;a:8]:[c:9]:[c:10]2:[#7;a:11]:[c:12]:[#7;a:13]:[#7;a:14]:2:1):[c:4]:[c:5]
37
[{"value": 37.0, "product": "C(C)(C)(C)OC(N(C=1C=2N(C(=CN1)C=1C=C3CCNC(C3=CC1)=O)N=CN2)C2=CC=C(C=C2)N2CCOCC2)=O", "details": "PERCENTYIELD", "is_desired": false}]
90
CELSIUS
8
HOUR
To a degassed solution of (4-morpholin-4-yl-phenyl)-(5-tributylstannanyl-[1,2,4]triazolo[1,5-a]pyrazin-8-yl)-carbamic acid tert-butyl ester (100 mg, 0.15 mmol) and 6-bromo-3,4-dihydro-2H-isoquinolin-1-one in DMF (1 mL) is added tetrakis(triphenylphosphine)palladium(0) (17 mg, 0.015 mmol) and the reaction mixture is sti...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Tin
null
c1cn2ncnc2cn1.c1ccc2c(c1)CCNC2
c1ccc2c(c1)CCNC2.c1cn2ncnc2cn1
c1ccccc1.C1COCC[NH]1.c1ccc2c(c1)CCNC2.c1cn2ncnc2cn1
HBr.Sn
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.CN(C)C=O
90
8
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1cnc(N(C(=O)OC(C)(C)C)c2ccc(N3CCOCC3)cc2)c2ncnn12.O=C1NCCc2cc(Br)ccc21>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.CN(C)C=O>CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1...
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7938c3edbdc54f608874a20b6cd31716
CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1)c1ncc(-c2ccc3c(c2)CCNC3=O)n2ncnc12>>O=C1NCCc2cc(-c3cnc(Nc4ccc(N5CCOCC5)cc4)c4ncnn34)ccc21
C(C)(C)(C)OC(N(C=1C=2N(C(=CN1)C=1C=C3CCNC(C3=CC1)=O)N=CN2)C2=CC=C(C=C2)N2CCOCC2)=O.C(=O)(C(F)(F)F)O>>N1(CCOCC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C3CCNC(C3=CC1)=O)N=CN2
CC(C)(C)OC(=O)[N:13]([c:12]1[n:11][cH:10][c:9](-[c:8]2[cH:7][c:6]3[c:33]([cH:32][cH:31]2)[C:2](=[O:1])[NH:3][CH2:4][CH2:5]3)[n:30]2[c:26]1[n:27][cH:28][n:29]2)[c:14]1[cH:15][cH:16][c:17]([N:18]2[CH2:19][CH2:20][O:21][CH2:22][CH2:23]2)[cH:24][cH:25]1>>[O:1]=[C:2]1[NH:3][CH2:4][CH2:5][c:6]2[cH:7][c:8](-[c:9]3[cH:10][n:11...
CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1)c1ncc(-c2ccc3c(c2)CCNC3=O)n2ncnc12
O=C1NCCc2cc(-c3cnc(Nc4ccc(N5CCOCC5)cc4)c4ncnn34)ccc21
null
C(Cl)Cl
null
Reduction
Boc amine deprotection
bbda4640db5f48af4538caded12fdadd56eacd6d4e5f7aefe46282d665df167e
a94b29c7264c852156fc1cdd4a0951a4fc26c06d0edc9e50c743825dbf79e3fd
O=C1NCCc2cc(-c3cnc(Nc4ccc(N5CCOCC5)cc4)c4ncnn34)ccc21
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1](-[c:2]1:[#7;a:3]:[c:4]:[c:5]:[#7;a:6]2:[#7;a:7]:[c:8]:[#7;a:9]:[c:10]:2:1)-[c:11](:[c:12]):[c:13]>>[c:12]:[c:11](-[NH;D2;+0:1]-[c:2]1:[#7;a:3]:[c:4]:[c:5]:[#7;a:6]2:[#7;a:7]:[c:8]:[#7;a:9]:[c:10]:2:1):[c:13]
null
[]
null
null
null
null
A solution of (4-morpholin-4-yl-phenyl)-[5-(1-oxo-1,2,3,4-tetrahydro-isoquinolin-6-yl)-[1,2,4]triazolo[1,5-a]pyrazin-8-yl]-carbamic acid tert-butyl ester (30 mg, 0.055 mmol) in a 1:1 mixture of TFA:DCM (1 drop of H2O), is stirred at room temperature for 2 hours. The solvent is removed in vacuo and the residue partition...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Secondary amine
null
null
c1ccc2c(c1)CCNC2.c1ccccc1.C1COCC[NH]1.c1cn2ncnc2cn1
HO-
C(Cl)Cl
null
null
CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1)c1ncc(-c2ccc3c(c2)CCNC3=O)n2ncnc12>C(Cl)Cl>O=C1NCCc2cc(-c3cnc(Nc4ccc(N5CCOCC5)cc4)c4ncnn34)ccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-53d975bc652a4e4b92204764fa281685
CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cn2)CC1.CC1(C)OB(c2ccc3c(c2)CNC3=O)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1>>CC(C)N1CCN(c2ccc(Nc3ncc(-c4ccc5c(c4)CNC5=O)n4ncnc34)cc2)CC1.N
CC1(OB(OC1(C)C)C=1C=C2CNC(C2=CC1)=O)C.CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2.BrC1=CN=C(C=2N1N=CN2)NC=2C=NC(=CC2)N2CCN(CC2)C(C)C>>N.C(C)(C)N1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C3CNC(C3=CC1)=O)N=CN2
Br[c:16]1[cH:15][n:14][c:13]([NH:12][c:11]2[cH:10][cH:9][c:8]([N:7]3[CH2:6][CH2:5][N:4]([CH:2]([CH3:1])[CH3:3])[CH2:35][CH2:34]3)n[cH:32]2)[c:31]2[n:27]1[n:28][cH:29][n:30]2.CC1(C)OB([c:17]2[cH:18][cH:19][c:20]3[c:21]([cH:22]2)[CH2:23][NH:24][C:25]3=[O:26])OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(=O)[NH2:36])c4)n4ncnc34)c[...
CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cn2)CC1.CC1(C)OB(c2ccc3c(c2)CNC3=O)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1
CC(C)N1CCN(c2ccc(Nc3ncc(-c4ccc5c(c4)CNC5=O)n4ncnc34)cc2)CC1.N
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O1CCOCC1.C(=O)([O-])[O-].[Na+].[Na+]
C-C Coupling
OtherReaction
a2d6d816881570f37f8a1f9df37f734d7c5a33d1c9b1b2ab51414b770206e0a5
96e5f3628c1bd4659dd3e9821904115decf673d0e8e42bb7900b7f521b084c51
O=C1NCc2cc(-c3cnc(Nc4ccc(N5CCNCC5)cc4)c4ncnn34)ccc21
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4](-[#7:5]-[c:6]2:[c:7]:[c:8]:[c;H0;D3;+0:9](-[#7:10](-[C:11])-[C:12]):n:[cH;D2;+0:13]:2):[c:14]2:[#7;a:15]:[c:16]:[#7;a:17]:[#7;a:18]:2:1.C-C1(-C)-O-B(-[c;H0;D3;+0:19](:[c:20]:[c:21]):[c:22]:[c:23])-O-C-1(-C)-C.C-N1-C-C-N(-c2:[cH;D2;+0:24]:c:c(-N-c3:n:c:c(-c4:c:s:c(-C(=O)-[NH2;D1;+...
53
[{"value": 53.0, "product": "C(C)(C)N1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C3CNC(C3=CC1)=O)N=CN2", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound may be prepared using methods as described for Compound 6, step 4 using 5-bromo-N-(6-(4-isopropylpiperazin-1-yl)pyridin-3-yl)-[1,2,4]triazolo[1,5-a]pyrazin-8-amine (0.6 g, 1.44 mmol), 5-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-2,3-dihydro-isoindol-1-one (0.56 g, 2.16 mmol) and Pd(PPh3)4 (0.416 g, 0....
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amide.Secondary amine.Tertiary amine.Tertiary amine.Boronic ester
null
c1ccncc1.c1cn2ncnc2cn1.B1OCCO1.c1ccc2c(c1)CNC2.C1CNCCN1.c1ccccc1.c1ccsc1.c1cn2ncnc2cn1
c1ccccc1.c1ccc2c(c1)CNC2.c1cn2ncnc2cn1
C1C[NH]CC[NH]1.c1ccccc1.c1ccc2c(c1)CNC2.c1cn2ncnc2cn1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1.C(=O)([O-])[O-].[Na+].[Na+]
null
null
CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cn2)CC1.CC1(C)OB(c2ccc3c(c2)CNC3=O)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1.C(=O)([...
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-15d03c4c681e44989f868d3ab7184f0b
O=Cc1cc([N+](=O)[O-])ccc1N1CCOCC1>>O=[N+]([O-])c1ccc(N2CCOCC2)c(CO)c1
N1(CCOCC1)C1=C(C=O)C=C(C=C1)[N+](=O)[O-].[BH4-].[Na+]>>N1(CCOCC1)C1=C(C=C(C=C1)[N+](=O)[O-])CO
[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]([N:8]2[CH2:9][CH2:10][O:11][CH2:12][CH2:13]2)[c:14]([CH:15]=[O:16])[cH:17]1>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]([N:8]2[CH2:9][CH2:10][O:11][CH2:12][CH2:13]2)[c:14]([CH2:15][OH:16])[cH:17]1
O=Cc1cc([N+](=O)[O-])ccc1N1CCOCC1
O=[N+]([O-])c1ccc(N2CCOCC2)c(CO)c1
null
null
CO
Reduction
Reduction of aldehydes and ketones to alcohols
e7895795cd3f75445716c94697823c5929dcd4b5344525875fe75d36bca2f9d7
21bb81d5469aaaca71ab12c186bea4016451717fad8780cf288858a7d8fbc55a
c1ccc(N2CCOCC2)cc1
[O;H0;D1;+0:1]=[CH;D2;+0:2]-[c:3](:[c:4]):[c:5]>>[OH;D1;+0:1]-[CH2;D2;+0:2]-[c:3](:[c:4]):[c:5]
107.7
[{"value": 107.7, "product": "N1(CCOCC1)C1=C(C=C(C=C1)[N+](=O)[O-])CO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
To a cooled (0° C.) solution of 2-morpholin-4-yl-5-nitro-benzaldehyde (0.8 g, 3.39 mmol) in MeOH (5 mL) is added NaBH4 (0.125 g, 3.39 mmol) and the reaction mixture is stirred at room temperature for 3 hours. After quenching the reaction with water, the solvent is removed in vacuo and the residue dissolved in ethyl ace...
10.6084/m9.figshare.5104873.v1
null
Aldehyde
Primary alcohol
null
null
c1ccccc1.C1COCC[NH]1
null
CO
null
3
O=Cc1cc([N+](=O)[O-])ccc1N1CCOCC1>CO>O=[N+]([O-])c1ccc(N2CCOCC2)c(CO)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-75019e1e3bef47e7aae77212098bbedc
O=[N+]([O-])c1ccc(N2CCOCC2)c(CO)c1>>Nc1ccc(N2CCOCC2)c(CO)c1
N1(CCOCC1)C1=C(C=C(C=C1)[N+](=O)[O-])CO>>NC=1C=CC(=C(C1)CO)N1CCOCC1
O=[N+:1]([O-])[c:2]1[cH:3][cH:4][c:5]([N:6]2[CH2:7][CH2:8][O:9][CH2:10][CH2:11]2)[c:12]([CH2:13][OH:14])[cH:15]1>>[NH2:1][c:2]1[cH:3][cH:4][c:5]([N:6]2[CH2:7][CH2:8][O:9][CH2:10][CH2:11]2)[c:12]([CH2:13][OH:14])[cH:15]1
O=[N+]([O-])c1ccc(N2CCOCC2)c(CO)c1
Nc1ccc(N2CCOCC2)c(CO)c1
null
null
C(C)O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc(N2CCOCC2)cc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
84.2
[{"value": 83.0, "product": "NC=1C=CC(=C(C1)CO)N1CCOCC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 84.2, "product": "NC=1C=CC(=C(C1)CO)N1CCOCC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
To a solution of (2-morpholin-4-yl-5-nitro-phenyl)-methanol (870 mg) in ethanol (40 mL) palladium hydroxide (87 mg) is added and the mixture is stirred in a Parr-apparatus under hydrogen pressure (10 bars) for 4 hours. The reaction mixture is filtrated over Celite 521, washed with ethanol and concentrated in vacuo to g...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1.C1COCC[NH]1
Other
C(C)O
null
4
O=[N+]([O-])c1ccc(N2CCOCC2)c(CO)c1>C(C)O>Nc1ccc(N2CCOCC2)c(CO)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c3d56357835e4c608cff369d74c8512d
Brc1ncc(Br)n2ncnc12.CC(C)(C)[SiH2]OC(C)(C)c1cc(N)ccc1N1CCOCC1>>CC(C)(C)[SiH2]OC(C)(C)c1cc(Nc2ncc(Br)n3ncnc23)ccc1N1CCOCC1
BrC1=CN=C(C=2N1N=CN2)Br.C(C)(C)(C)[SiH2]OC(C=1C=C(C=CC1N1CCOCC1)N)(C)C.C(C)N(C(C)C)C(C)C>>BrC1=CN=C(C=2N1N=CN2)NC2=CC(=C(C=C2)N2CCOCC2)C(O[SiH2]C(C)(C)C)(C)C
Br[c:14]1[n:15][cH:16][c:17]([Br:18])[n:19]2[n:20][cH:21][n:22][c:23]12.[CH3:1][C:2]([CH3:3])([CH3:4])[SiH2:5][O:6][C:7]([CH3:8])([CH3:9])[c:10]1[cH:11][c:12]([NH2:13])[cH:24][cH:25][c:26]1[N:27]1[CH2:28][CH2:29][O:30][CH2:31][CH2:32]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[SiH2:5][O:6][C:7]([CH3:8])([CH3:9])[c:10]1[cH:11][c:...
Brc1ncc(Br)n2ncnc12.CC(C)(C)[SiH2]OC(C)(C)c1cc(N)ccc1N1CCOCC1
CC(C)(C)[SiH2]OC(C)(C)c1cc(Nc2ncc(Br)n3ncnc23)ccc1N1CCOCC1
null
null
CC(C)O
Heteroatom Alkylation and Arylation
N-arylation (Buchwald-Hartwig/Ullmann-Goldberg)
aecfb0ede2c5d7901fea69101287828edf21f7a6e48b6ff83fe43de0688f1ef1
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1cn2ncnc2c(Nc2ccc(N3CCOCC3)cc2)n1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:1.[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[c:12]:[c:11](-[NH;D2;+0:10]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:1):[c:13]
46
[{"value": 46.0, "product": "BrC1=CN=C(C=2N1N=CN2)NC2=CC(=C(C=C2)N2CCOCC2)C(O[SiH2]C(C)(C)C)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 45.7, "product": "BrC1=CN=C(C=2N1N=CN2)NC2=CC(=C(C=C2)N2CCOCC2)C(O[SiH2]C(C)(C)C)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 5,8-dibromo-[1,2,4]triazolo[1,5-a]pyrazine (0.391 g, 1.41 mmol), 3-(tert-butyl-dimethyl-silanyloxymethyl)-4-morpholin-4-yl-phenylamine (0.5 g, 1.55 mmol) and N-ethyldiisopropyl-amine (0.27 mL, 1.55 mmol) is heated at 90° C. in 2-propanol (10 mL) for 8 hours. The reaction mixture is evaporated to dryness an...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1cn2ncnc2cn1
c1cn2ncnc2cn1
c1ccccc1.c1cn2ncnc2cn1.C1COCC[NH]1
HBr
CC(C)O
null
null
Brc1ncc(Br)n2ncnc12.CC(C)(C)[SiH2]OC(C)(C)c1cc(N)ccc1N1CCOCC1>CC(C)O>CC(C)(C)[SiH2]OC(C)(C)c1cc(Nc2ncc(Br)n3ncnc23)ccc1N1CCOCC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-84ec7188b62045c095ea3d6a40c8ef00
CC1(C)OB(c2cn[nH]c2)OC1(C)C.OCc1cc(Nc2ncc(Br)n3ncnc23)ccc1N1CCOCC1>>OCc1cc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)ccc1N1CCOCC1
CC1(OB(OC1(C)C)C=1C=NNC1)C.CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2.BrC1=CN=C(C=2N1N=CN2)NC=2C=CC(=C(C2)CO)N2CCOCC2>>N1N=CC(=C1)C1=CN=C(C=2N1N=CN2)NC=2C=CC(=C(C2)CO)N2CCOCC2
CC1(C)OB([c:11]2[cH:12][n:13][nH:14][cH:15]2)OC1(C)C.Br[c:10]1[cH:9][n:8][c:7]([NH:6][c:5]2[cH:4][c:3]([CH2:2][OH:1])[c:23]([N:24]3[CH2:25][CH2:26][O:27][CH2:28][CH2:29]3)[cH:22][cH:21]2)[c:20]2[n:16]1[n:17][cH:18][n:19]2>>[OH:1][CH2:2][c:3]1[cH:4][c:5]([NH:6][c:7]2[n:8][cH:9][c:10](-[c:11]3[cH:12][n:13][nH:14][cH:15]3...
CC1(C)OB(c2cn[nH]c2)OC1(C)C.OCc1cc(Nc2ncc(Br)n3ncnc23)ccc1N1CCOCC1
OCc1cc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)ccc1N1CCOCC1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O1CCOCC1.C(=O)([O-])[O-].[Na+].[Na+]
C-C Coupling
Suzuki coupling with boronic esters
3b077e58a8068174133a7eecad35957570f9290725408c31a955826b02d2e470
b42efb3b6a7742d5af594c6a3031e487327e58e9f8c2f428ee68996c98377910
c1nc2c(Nc3ccc(N4CCOCC4)cc3)ncc(-c3cn[nH]c3)n2n1
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1.C-C1(-C)-O-B(-[c;H0;D3;+0:10]2:[c:11]:[#7;a:12]:[#7;a:13]:[c:14]:2)-O-C-1(-C)-C>>[#7;a:12]1:[#7;a:13]:[c:14]:[c;H0;D3;+0:10](-[c;H0;D3;+0:1]2:[c:2]:[#7;a:3]:[c:4]:[c:5]3:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:3:2):[c:11]:1
12
[{"value": 12.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound may be prepared using methods as described for Compound 6, step 4 using [5-(5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-ylamino)-2-morpholin-4-yl-phenyl]-methanol (85 mg, 0.21 mmol), 4-(4,4,5,5-tetramethyl-[1,3,2]dioxa-borolan-2-yl)-1H-pyrazole (81 mg, 0.42 mmol) and Pd(PPh3)4 (60 mg, 0.052 mmol) in 1.5M Na2C...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic ester
null
B1OCCO1.c1cn[nH]c1.c1cn2ncnc2cn1
c1cn[nH]c1.c1cn2ncnc2cn1
c1ccccc1.c1cn[nH]c1.c1cn2ncnc2cn1.C1COCC[NH]1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1.C(=O)([O-])[O-].[Na+].[Na+]
null
null
CC1(C)OB(c2cn[nH]c2)OC1(C)C.OCc1cc(Nc2ncc(Br)n3ncnc23)ccc1N1CCOCC1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1.C(=O)([O-])[O-].[Na+].[Na+]>OCc1cc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)ccc1N1CCOC...
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a066fb1722274b7c9b1147bd17cfb52b
Brc1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12.CC1(C)OB(c2csc3ccccc23)OC1(C)C>>c1ccc2c(-c3cnc(Nc4ccc(N5CCOCC5)cc4)c4ncnn34)csc2c1
BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2CCOCC2.CC1(OB(OC1(C)C)C=1C2=C(SC1)C=CC=C2)C>>S1C2=C(C(=C1)C1=CN=C(C=3N1N=CN3)NC3=CC=C(C=C3)N3CCOCC3)C=CC=C2
Br[c:6]1[cH:7][n:8][c:9]([NH:10][c:11]2[cH:12][cH:13][c:14]([N:15]3[CH2:16][CH2:17][O:18][CH2:19][CH2:20]3)[cH:21][cH:22]2)[c:23]2[n:24][cH:25][n:26][n:27]12.CC1(C)OB([c:5]2[c:4]3[cH:3][cH:2][cH:1][cH:31][c:30]3[s:29][cH:28]2)OC1(C)C>>[cH:1]1[cH:2][cH:3][c:4]2[c:5](-[c:6]3[cH:7][n:8][c:9]([NH:10][c:11]4[cH:12][cH:13][c...
Brc1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12.CC1(C)OB(c2csc3ccccc23)OC1(C)C
c1ccc2c(-c3cnc(Nc4ccc(N5CCOCC5)cc4)c4ncnn34)csc2c1
null
null
null
C-C Coupling
Suzuki coupling with boronic esters
b93680bb40a0e9e2c1d4273451dc351a647432fa5a851c052732cedf7ebf5184
b42efb3b6a7742d5af594c6a3031e487327e58e9f8c2f428ee68996c98377910
c1ccc2c(-c3cnc(Nc4ccc(N5CCOCC5)cc4)c4ncnn34)csc2c1
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1.C-C1(-C)-O-B(-[c;H0;D3;+0:10]2:[c:11]:[#16;a:12]:[c:13](:[c:14]):[c:15]:2:[c:16])-O-C-1(-C)-C>>[c:14]:[c:13]1:[#16;a:12]:[c:11]:[c;H0;D3;+0:10](-[c;H0;D3;+0:1]2:[c:2]:[#7;a:3]:[c:4]:[c:5]3:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:3:2):[c:15]:1:...
null
[]
null
null
null
null
This compound may be prepared using methods as described for Compound 120, using (5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-yl)-(4-morpholin-4-ylphenyl)amine and 4,4,5,5-tetramethyl-2-benzo[b]thiophen-3-yl-[1,3,2]dioxaborolane in step 4. LCMS: Rt 0.84 min (95%), m/z (ESI) 402 (M+H)+. Conditions: See reaction.notes.proced...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic ester
null
c1cn2ncnc2cn1.B1OCCO1.c1ccc2sccc2c1
c1cn2ncnc2cn1.c1ccc2sccc2c1
c1ccccc1.C1COCC[NH]1.c1cn2ncnc2cn1.c1ccc2sccc2c1
HBr.B
null
null
null
Brc1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12.CC1(C)OB(c2csc3ccccc23)OC1(C)C>>c1ccc2c(-c3cnc(Nc4ccc(N5CCOCC5)cc4)c4ncnn34)csc2c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-672580c563064a18b763e72fd568a784
Brc1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12.CC1(C)OB(c2ccsc2)OC1(C)C>>c1nc2c(Nc3ccc(N4CCOCC4)cc3)ncc(-c3ccsc3)n2n1
BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2CCOCC2.CC1(OB(OC1(C)C)C1=CSC=C1)C>>N1(CCOCC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C1=CSC=C1)N=CN2
Br[c:20]1[cH:19][n:18][c:4]([NH:5][c:6]2[cH:7][cH:8][c:9]([N:10]3[CH2:11][CH2:12][O:13][CH2:14][CH2:15]3)[cH:16][cH:17]2)[c:3]2[n:2][cH:1][n:27][n:26]21.CC1(C)OB([c:21]2[cH:22][cH:23][s:24][cH:25]2)OC1(C)C>>[cH:1]1[n:2][c:3]2[c:4]([NH:5][c:6]3[cH:7][cH:8][c:9]([N:10]4[CH2:11][CH2:12][O:13][CH2:14][CH2:15]4)[cH:16][cH:1...
Brc1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12.CC1(C)OB(c2ccsc2)OC1(C)C
c1nc2c(Nc3ccc(N4CCOCC4)cc3)ncc(-c3ccsc3)n2n1
null
null
null
C-C Coupling
Suzuki coupling with boronic esters
791f73e9e8c7588b7846191c9fedfcf6e2595c90e46d286b94f30804a763a2ec
b42efb3b6a7742d5af594c6a3031e487327e58e9f8c2f428ee68996c98377910
c1nc2c(Nc3ccc(N4CCOCC4)cc3)ncc(-c3ccsc3)n2n1
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1.C-C1(-C)-O-B(-[c;H0;D3;+0:10]2:[c:11]:[c:12]:[#16;a:13]:[c:14]:2)-O-C-1(-C)-C>>[#16;a:13]1:[c:12]:[c:11]:[c;H0;D3;+0:10](-[c;H0;D3;+0:1]2:[c:2]:[#7;a:3]:[c:4]:[c:5]3:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:3:2):[c:14]:1
null
[]
null
null
null
null
This compound may be prepared using methods as described for Compound 120, using (5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-yl)-(4-morpholin-4-ylphenyl)amine and 4,4,5,5-tetramethyl-2-thiophen-3-yl-[1,3,2]dioxaborolane in step 4. LCMS: Rt 1.19 min (95%), m/z (ESI) 379 (M+H)+. Conditions: See reaction.notes.procedure_deta...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic ester
null
c1cn2ncnc2cn1.B1OCCO1.c1ccsc1
c1cn2ncnc2cn1.c1ccsc1
c1ccccc1.C1COCC[NH]1.c1cn2ncnc2cn1.c1ccsc1
HBr.B
null
null
null
Brc1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12.CC1(C)OB(c2ccsc2)OC1(C)C>>c1nc2c(Nc3ccc(N4CCOCC4)cc3)ncc(-c3ccsc3)n2n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-396a2a55c1a547f69c1569621ac6bcca
Brc1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12.CCc1c(B2OC(C)(C)C(C)(C)O2)cnn1C1CCCCO1>>CCc1[nH]ncc1-c1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12
CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2.C(=O)([O-])[O-].[Na+].[Na+].C(C)C1=C(C=NN1C1OCCCC1)B1OC(C(O1)(C)C)(C)C.C(C)C1=NN(C=C1B1OC(C(O1)(C)C)(C)C)C1OCCCC1.BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2CCOCC2>>C(C)C1=C(C=NN1)C1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2CCOCC2
Br[c:8]1[cH:9][n:10][c:11]([NH:12][c:13]2[cH:14][cH:15][c:16]([N:17]3[CH2:18][CH2:19][O:20][CH2:21][CH2:22]3)[cH:23][cH:24]2)[c:25]2[n:26][cH:27][n:28][n:29]12.CC1(C)OB([c:7]2[c:3]([CH2:2][CH3:1])[n:4](C3CCCCO3)[n:5][cH:6]2)OC1(C)C>>[CH3:1][CH2:2][c:3]1[nH:4][n:5][cH:6][c:7]1-[c:8]1[cH:9][n:10][c:11]([NH:12][c:13]2[cH:...
Brc1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12.CCc1c(B2OC(C)(C)C(C)(C)O2)cnn1C1CCCCO1
CCc1[nH]ncc1-c1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O1CCOCC1
C-C Coupling
OtherReaction
5b250e4178d9f7ec19c8f75544930eff90278ccea3ebf86411859b7895245136
664bb683b7d04c49fddf80239ea7ce0c421519efd3bdfdeb0820befa736cf196
c1nc2c(Nc3ccc(N4CCOCC4)cc3)ncc(-c3cn[nH]c3)n2n1
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1.C-C1(-C)-O-B(-[c;H0;D3;+0:10]2:[c:11]:[#7;a:12]:[n;H0;D3;+0:13](-C3-C-C-C-C-O-3):[c:14]:2-[C:15])-O-C-1(-C)-C>>[C:15]-[c:14]1:[nH;D2;+0:13]:[#7;a:12]:[c:11]:[c;H0;D3;+0:10]:1-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#...
null
[]
null
null
null
null
This compound may be prepared using methods as described for Compound 6, step 4 using (5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-yl)-(4-morpholin-4-yl-phenyl)-amine (0.032 g, 0.085 mmol), 5-ethyl-1-(tetrahydro-pyran-2-yl)-4-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-1H-pyrazole and 3-ethyl-1-(tetrahydro-pyran-2-yl)-4...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ether.Boronic ester
null
c1cn2ncnc2cn1.B1OCCO1.c1c[nH]nc1.C1CCOCC1
c1cn[nH]c1.c1cn2ncnc2cn1
c1cn[nH]c1.c1ccccc1.C1COCC[NH]1.c1cn2ncnc2cn1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1
null
null
Brc1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12.CCc1c(B2OC(C)(C)C(C)(C)O2)cnn1C1CCCCO1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1>CCc1[nH]ncc1-c1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-bec95c032eb84b4ca0472d157d283fe2
CCc1nn(C2CCCCO2)cc1-c1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12>>CCc1[nH]ncc1-c1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12
C(C)C1=C(C=NN1C1OCCCC1)C1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2CCOCC2.C(C)C1=NN(C=C1C1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2CCOCC2)C2OCCCC2.Cl>>C(C)C1=C(C=NN1)C1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2CCOCC2
C1CCC([n:5]2[n:4][c:3]([CH2:2][CH3:1])[c:7](-[c:8]3[cH:9][n:10][c:11]([NH:12][c:13]4[cH:14][cH:15][c:16]([N:17]5[CH2:18][CH2:19][O:20][CH2:21][CH2:22]5)[cH:23][cH:24]4)[c:25]4[n:26][cH:27][n:28][n:29]34)[cH:6]2)OC1>>[CH3:1][CH2:2][c:3]1[nH:4][n:5][cH:6][c:7]1-[c:8]1[cH:9][n:10][c:11]([NH:12][c:13]2[cH:14][cH:15][c:16](...
CCc1nn(C2CCCCO2)cc1-c1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12
CCc1[nH]ncc1-c1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12
null
null
CO
Reduction
OtherReaction
961a72974526db3621ed05df5cf40c54af32f87acb02ef9960ca6098e4d5b0ab
84394d34c591024a84d9393eb3e8adb8ada5a6225c3abafc4dae9aedd4568be4
c1nc2c(Nc3ccc(N4CCOCC4)cc3)ncc(-c3cn[nH]c3)n2n1
[C:1]-[c:2]1:[c:3]:[c:4]:[n;H0;D3;+0:5](-C2-C-C-C-C-O-2):[n;H0;D2;+0:6]:1>>[C:1]-[c:2]1:[c:3]:[c:4]:[n;H0;D2;+0:5]:[nH;D2;+0:6]:1
17
[{"value": 17.0, "product": "C(C)C1=C(C=NN1)C1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2CCOCC2", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of {5-[5-ethyl-1-(tetrahydro-pyran-2-yl)-1H-pyrazol-4-yl]-[1,2,4]triazolo[1,5-a]pyrazin-8-yl}-(4-morpholin-4-yl-phenyl)-amine and {5-[3-ethyl-1-(tetrahydro-pyran-2-yl)-1H-pyrazol-4-yl]-[1,2,4]triazolo[1,5-a]pyrazin-8-yl}-(4-morpholin-4-yl-phenyl)-amine (40 mg, 0.077 mmol) and conc. HCl (0.3 mL) in MeOH (10 m...
10.6084/m9.figshare.5104873.v1
null
Ether
null
C1CCOCC1.c1cn[nH]c1
c1cn[nH]c1
c1cn[nH]c1.c1ccccc1.C1COCC[NH]1.c1cn2ncnc2cn1
HO-
CO
null
null
CCc1nn(C2CCCCO2)cc1-c1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12>CO>CCc1[nH]ncc1-c1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4c857d3926b7406ebf93ef0b47bf93d2
CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1)c1ncc(Br)n2ncnc12.CC1(C)OB(c2ccc3c(c2)S(=O)(=O)NC3=O)OC1(C)C>>CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1)c1ncc(-c2ccc3c(c2)S(=O)(=O)NC3=O)n2ncnc12
C(=O)([O-])[O-].[Na+].[Na+].CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2.C(C)(C)(C)OC(N(C1=CC=C(C=C1)N1CCOCC1)C=1C=2N(C(=CN1)Br)N=CN2)=O.O=S1(NC(C2=C1C=C(C=C2)B2OC(C(O2)(C)C)(C)C)=O)=O>>C(C)(C)(C)OC(N(C=1C=2N(C(=CN1)C1=CC3=C(C(NS3(=O)=O)=O)C=C1)N=CN2)C2=CC=C(C=C2)N2CCOCC2)=O
Br[c:24]1[cH:23][n:22][c:21]([N:8]([C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[c:9]2[cH:10][cH:11][c:12]([N:13]3[CH2:14][CH2:15][O:16][CH2:17][CH2:18]3)[cH:19][cH:20]2)[c:41]2[n:37]1[n:38][cH:39][n:40]2.CC1(C)OB([c:25]2[cH:26][cH:27][c:28]3[c:29]([cH:30]2)[S:31](=[O:32])(=[O:33])[NH:34][C:35]3=[O:36])OC1(C)C>>[CH...
CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1)c1ncc(Br)n2ncnc12.CC1(C)OB(c2ccc3c(c2)S(=O)(=O)NC3=O)OC1(C)C
CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1)c1ncc(-c2ccc3c(c2)S(=O)(=O)NC3=O)n2ncnc12
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O1CCOCC1
C-C Coupling
Suzuki coupling with boronic esters
a4e44fbcfebb2e9ed792a442fe98ba6e4e5c8972cb98fc27d617b9afb5655b91
b42efb3b6a7742d5af594c6a3031e487327e58e9f8c2f428ee68996c98377910
O=C1NS(=O)(=O)c2cc(-c3cnc(Nc4ccc(N5CCOCC5)cc4)c4ncnn34)ccc21
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1.C-C1(-C)-O-B(-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]-[#16:15])-O-C-1(-C)-C>>[#16:15]-[c:14]:[c:13]:[c;H0;D3;+0:10](-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1):[c:11]:[c:12]
44
[{"value": 44.0, "product": "C(C)(C)(C)OC(N(C=1C=2N(C(=CN1)C1=CC3=C(C(NS3(=O)=O)=O)C=C1)N=CN2)C2=CC=C(C=C2)N2CCOCC2)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 43.8, "product": "C(C)(C)(C)OC(N(C=1C=2N(C(=CN1)C1=CC3=C(C(NS3(=O)=O)=O)C=C1)N=CN2)C2=CC=C(C=C2)N2CCOCC2)=O", "details": "CALCULATEDPERCENTY...
null
null
null
null
This compound may be prepared using methods as described for Compound 6, step 4 using (5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-yl)-(4-morpholin-4-yl-phenyl)-carbamic acid tert-butyl ester (170 mg, 0.36 mmol), 1,1-dioxo-6-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-1,2-dihydro-1λ6-benzo[d]isothiazol-3-one (374 mg, 0....
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic ester
null
c1cn2ncnc2cn1.B1OCCO1.c1ccc2c(c1)CNS2
c1ccc2c(c1)CNS2.c1cn2ncnc2cn1
c1ccccc1.C1COCC[NH]1.c1ccc2c(c1)CNS2.c1cn2ncnc2cn1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1
null
null
CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1)c1ncc(Br)n2ncnc12.CC1(C)OB(c2ccc3c(c2)S(=O)(=O)NC3=O)OC1(C)C>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1>CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1)c1ncc(-c2...
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2a87de850dfd4c0298869c44948ccf9e
CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1)c1ncc(-c2ccc3c(c2)S(=O)(=O)NC3=O)n2ncnc12>>O=C1NS(=O)(=O)c2cc(-c3cnc(Nc4ccc(N5CCOCC5)cc4)c4ncnn34)ccc21
C(C)(C)(C)OC(N(C=1C=2N(C(=CN1)C1=CC3=C(C(NS3(=O)=O)=O)C=C1)N=CN2)C2=CC=C(C=C2)N2CCOCC2)=O>>N1(CCOCC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C1=CC3=C(C(NS3(=O)=O)=O)C=C1)N=CN2
CC(C)(C)OC(=O)[N:14]([c:13]1[n:12][cH:11][c:10](-[c:9]2[cH:8][c:7]3[c:34]([cH:33][cH:32]2)[C:2](=[O:1])[NH:3][S:4]3(=[O:5])=[O:6])[n:31]2[c:27]1[n:28][cH:29][n:30]2)[c:15]1[cH:16][cH:17][c:18]([N:19]2[CH2:20][CH2:21][O:22][CH2:23][CH2:24]2)[cH:25][cH:26]1>>[O:1]=[C:2]1[NH:3][S:4](=[O:5])(=[O:6])[c:7]2[cH:8][c:9](-[c:10...
CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1)c1ncc(-c2ccc3c(c2)S(=O)(=O)NC3=O)n2ncnc12
O=C1NS(=O)(=O)c2cc(-c3cnc(Nc4ccc(N5CCOCC5)cc4)c4ncnn34)ccc21
null
null
Cl.O1CCOCC1
Reduction
Boc amine deprotection
bbda4640db5f48af4538caded12fdadd56eacd6d4e5f7aefe46282d665df167e
a94b29c7264c852156fc1cdd4a0951a4fc26c06d0edc9e50c743825dbf79e3fd
O=C1NS(=O)(=O)c2cc(-c3cnc(Nc4ccc(N5CCOCC5)cc4)c4ncnn34)ccc21
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1](-[c:2]1:[#7;a:3]:[c:4]:[c:5]:[#7;a:6]2:[#7;a:7]:[c:8]:[#7;a:9]:[c:10]:2:1)-[c:11](:[c:12]):[c:13]>>[c:12]:[c:11](-[NH;D2;+0:1]-[c:2]1:[#7;a:3]:[c:4]:[c:5]:[#7;a:6]2:[#7;a:7]:[c:8]:[#7;a:9]:[c:10]:2:1):[c:13]
101.7
[{"value": 100.0, "product": "N1(CCOCC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C1=CC3=C(C(NS3(=O)=O)=O)C=C1)N=CN2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 101.7, "product": "N1(CCOCC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C1=CC3=C(C(NS3(=O)=O)=O)C=C1)N=CN2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
A suspension of (4-morpholin-4-yl-phenyl)-[5-(1,1,3-trioxo-2,3-dihydro-1H-1 λ6-benzo[d]isothiazol-6-yl)-[1,2,4]triazolo[1,5-a]pyrazin-8-yl]-carbamic acid tert-butyl ester (100 mg, 0.173 mmol) in 4M HCl (2.5 mL) in dioxane is stirred at room temperature for 2 hours. The solvent is removed under vacuum and the residue is...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Secondary amine
null
null
c1ccc2c(c1)CNS2.c1ccccc1.C1COCC[NH]1.c1cn2ncnc2cn1
HO-
Cl.O1CCOCC1
null
2
CC(C)(C)OC(=O)N(c1ccc(N2CCOCC2)cc1)c1ncc(-c2ccc3c(c2)S(=O)(=O)NC3=O)n2ncnc12>Cl.O1CCOCC1>O=C1NS(=O)(=O)c2cc(-c3cnc(Nc4ccc(N5CCOCC5)cc4)c4ncnn34)ccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9b56b59d5fa145af9eed651afa727787
NC(=O)c1cc(B(O)O)cs1.c1nc2c(Nc3ccc(N4CCN(CC5CC5)CC4)cc3)ncc(-c3cn[nH]c3)n2n1>>NC(=O)c1cc(-c2cnc(Nc3ccc(N4CCN(CC5CC5)CC4)cc3)c3ncnn23)cs1
C1(CC1)CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=NNC1)N=CN2.NC(=O)C=1SC=C(C1)B(O)O>>C1(CC1)CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2
OB(O)[c:6]1[cH:5][c:4]([C:2]([NH2:1])=[O:3])[s:34][cH:33]1.c1n[nH]cc1-[c:7]1[cH:8][n:9][c:10]([NH:11][c:12]2[cH:13][cH:14][c:15]([N:16]3[CH2:17][CH2:18][N:19]([CH2:20][CH:21]4[CH2:22][CH2:23]4)[CH2:24][CH2:25]3)[cH:26][cH:27]2)[c:28]2[n:29][cH:30][n:31][n:32]12>>[NH2:1][C:2](=[O:3])[c:4]1[cH:5][c:6](-[c:7]2[cH:8][n:9][...
NC(=O)c1cc(B(O)O)cs1.c1nc2c(Nc3ccc(N4CCN(CC5CC5)CC4)cc3)ncc(-c3cn[nH]c3)n2n1
NC(=O)c1cc(-c2cnc(Nc3ccc(N4CCN(CC5CC5)CC4)cc3)c3ncnn23)cs1
null
null
null
C-C Coupling
OtherReaction
f3b9026c2e0fca3f66449ae83278e72e26246a4e0c9e12eb550a3525259554d6
fb7ad422d905bdc265298a43c871eec14eab0c8cca46cc3d1bd494f2a986d765
c1nc2c(Nc3ccc(N4CCN(CC5CC5)CC4)cc3)ncc(-c3ccsc3)n2n1
O-B(-O)-[c;H0;D3;+0:1]1:[c:2]:[#16;a:3]:[c:4](-[C:5](-[N;D1;H2:6])=[O;D1;H0:7]):[c:8]:1.[#7;a:9]1:[c:10]:[#7;a:11]:[#7;a:12]2:[c:13]:1:[c:14]:[#7;a:15]:[c:16]:[c;H0;D3;+0:17]:2-c1:c:[nH]:n:c:1>>[N;D1;H2:6]-[C:5](=[O;D1;H0:7])-[c:4]1:[#16;a:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:17]2:[c:16]:[#7;a:15]:[c:14]:[c:13]3:[#7;a:...
null
[]
null
null
null
null
This compound may be prepared using methods as described for Compound 46, using 2-(aminocarbonyl)thiophene-4-boronic acid. LCMS: Rt=0.93 (95%), m/z (ESI) 475 (M+H)+. Conditions: See reaction.notes.procedure_details. Workup: This compound may be prepared
10.6084/m9.figshare.5104873.v1
null
Boronic acid
null
c1ccsc1.c1cn[nH]c1.c1cn2ncnc2cn1
c1ccsc1.c1cn2ncnc2cn1
c1ccsc1.c1ccccc1.C1C[NH]CC[NH]1.C1CC1.c1cn2ncnc2cn1
HO-.B
null
null
null
NC(=O)c1cc(B(O)O)cs1.c1nc2c(Nc3ccc(N4CCN(CC5CC5)CC4)cc3)ncc(-c3cn[nH]c3)n2n1>>NC(=O)c1cc(-c2cnc(Nc3ccc(N4CCN(CC5CC5)CC4)cc3)c3ncnn23)cs1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1efc6fe587264f8aaf7606db9287f461
Brc1cnc(Nc2ccc(N3CCN(C4CC4)CC3)cc2)c2ncnn12.c1nc2c(Nc3ccc(N4CCN(CC5CC5)CC4)cc3)ncc(-c3cn[nH]c3)n2n1>>c1nc2c(Nc3ccc(N4CCN(C5CC5)CC4)cc3)ncc(-c3cn[nH]c3)n2n1
C1(CC1)CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=NNC1)N=CN2.BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2CCN(CC2)C2CC2>>C1(CC1)N1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=NNC1)N=CN2
Brc1cnc(Nc2ccc(N3CCN([CH:14]4[CH2:15][CH2:16]4)CC3)cc2)c2ncnn12.C1CC1C[N:13]1[CH2:12][CH2:11][N:10]([c:9]2[cH:8][cH:7][c:6]([NH:5][c:4]3[c:3]4[n:2][cH:1][n:30][n:29]4[c:23](-[c:24]4[cH:25][n:26][nH:27][cH:28]4)[cH:22][n:21]3)[cH:20][cH:19]2)[CH2:18][CH2:17]1>>[cH:1]1[n:2][c:3]2[c:4]([NH:5][c:6]3[cH:7][cH:8][c:9]([N:10]...
Brc1cnc(Nc2ccc(N3CCN(C4CC4)CC3)cc2)c2ncnn12.c1nc2c(Nc3ccc(N4CCN(CC5CC5)CC4)cc3)ncc(-c3cn[nH]c3)n2n1
c1nc2c(Nc3ccc(N4CCN(C5CC5)CC4)cc3)ncc(-c3cn[nH]c3)n2n1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
dee39114e4673f33fbc41f563b9534d440103232ec7deedb605e56fdd0259127
620797dd8280f68fb96af89f30cfa19ffb92b9594066c67b5bfa02ac48fff79f
c1nc2c(Nc3ccc(N4CCN(C5CC5)CC4)cc3)ncc(-c3cn[nH]c3)n2n1
Br-c1:c:n:c(-N-c2:c:c:c(-N3-C-C-N(-[CH;D3;+0:1]4-[C:2]-[C:3]-4)-C-C-3):c:c:2):c2:n:c:n:n:1:2.C1-C-C-1-C-[N;H0;D3;+0:4]1-[C:5]-[C:6]-[#7:7]-[C:8]-[C:9]-1>>[#7:7]1-[C:6]-[C:5]-[N;H0;D3;+0:4](-[CH;D3;+0:1]2-[C:2]-[C:3]-2)-[C:9]-[C:8]-1
null
[]
null
null
null
null
This compound may be prepared using methods as described for Compound 46, using (5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-yl)-[4-(4-cyclopropylpiperazin-1-yl)-phenyl]amine. LCMS: Rt=0.84 (95%), m/z (ESI) 402 (M+H)+. Conditions: See reaction.notes.procedure_details. Workup: This compound may be prepared
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Secondary amine.Tertiary amine.Tertiary amine.Tertiary amine
Tertiary amine
c1ccccc1.C1CNCCN1.C1CC1.c1cn2ncnc2cn1.C1CC1.C1C[NH]CC[NH]1
C1C[NH]CC[NH]1.C1CC1
c1ccccc1.C1C[NH]CC[NH]1.C1CC1.c1cn2ncnc2cn1.c1cn[nH]c1
HBr
null
null
null
Brc1cnc(Nc2ccc(N3CCN(C4CC4)CC3)cc2)c2ncnn12.c1nc2c(Nc3ccc(N4CCN(CC5CC5)CC4)cc3)ncc(-c3cn[nH]c3)n2n1>>c1nc2c(Nc3ccc(N4CCN(C5CC5)CC4)cc3)ncc(-c3cn[nH]c3)n2n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-458f93ff7bf64ce7b249c7fe30a69a34
O=C(N1CCC(c2ccc([N+](=O)[O-])cc2)CC1)C(F)(F)F>>O=[N+]([O-])c1ccc(C2CCN(CC(F)(F)F)CC2)cc1
N#N.[BH4-].[Na+].FC(C(=O)N1CCC(CC1)C1=CC=C(C=C1)[N+](=O)[O-])(F)F.II>>FC(CN1CCC(CC1)C1=CC=C(C=C1)[N+](=O)[O-])(F)F
O=[C:12]([N:11]1[CH2:10][CH2:9][CH:8]([c:7]2[cH:6][cH:5][c:4]([N+:2](=[O:1])[O-:3])[cH:20][cH:19]2)[CH2:18][CH2:17]1)[C:13]([F:14])([F:15])[F:16]>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]([CH:8]2[CH2:9][CH2:10][N:11]([CH2:12][C:13]([F:14])([F:15])[F:16])[CH2:17][CH2:18]2)[cH:19][cH:20]1
O=C(N1CCC(c2ccc([N+](=O)[O-])cc2)CC1)C(F)(F)F
O=[N+]([O-])c1ccc(C2CCN(CC(F)(F)F)CC2)cc1
null
null
C1CCOC1
Reduction
Reduction of tertiary amides to amines
f74c5a050b269ec4da3871c266f01344b7447381f47cda744f8b1e9c225ae62d
c8f3c617792f7a4fae96b8a97dc0ce23461ab85d8a738fe6caacff776ef51ffa
c1ccc(C2CCNCC2)cc1
O=[C;H0;D3;+0:1](-[#7:2](-[C:3])-[C:4])-[C:5](-[F;D1;H0:6])(-[F;D1;H0:7])-[F;D1;H0:8]>>[C:3]-[#7:2](-[CH2;D2;+0:1]-[C:5](-[F;D1;H0:6])(-[F;D1;H0:7])-[F;D1;H0:8])-[C:4]
null
[]
0
CELSIUS
null
null
A solution of 1-trifluoroacetyl-4-(4-nitrophenyl)piperidine (1.42 g, 4.7 mmol) in THF (15 mL) is stirred in 25 mL 2-necked flask fitted with a condenser and pressure-equalizing addition funnel. The system is flushed with N2, NaBH4 (210 mg, 5.6 mmol) is added and the flask is cooled to 0° C. A solution of iodine (600 mg...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide
null
null
null
c1ccccc1.C1CC[NH]CC1
Other
C1CCOC1
0
null
O=C(N1CCC(c2ccc([N+](=O)[O-])cc2)CC1)C(F)(F)F>C1CCOC1>O=[N+]([O-])c1ccc(C2CCN(CC(F)(F)F)CC2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ceaf160cdc434884bdc4d842b0127abb
O=[N+]([O-])c1ccc(C2CCN(CC(F)(F)F)CC2)cc1>>O=CNc1ccc(C2CCN(CC(F)(F)F)CC2)cc1
C(=O)[O-].[NH4+].FC(CN1CCC(CC1)C1=CC=C(C=C1)[N+](=O)[O-])(F)F.C(=O)[O-].[NH4+]>>FC(CN1CCC(CC1)C1=CC=C(C=C1)NC=O)(F)F
O=[N+:3]([O-])[c:4]1[cH:5][cH:6][c:7]([CH:8]2[CH2:9][CH2:10][N:11]([CH2:12][C:13]([F:14])([F:15])[F:16])[CH2:17][CH2:18]2)[cH:19][cH:20]1>>[O:1]=[CH:2][NH:3][c:4]1[cH:5][cH:6][c:7]([CH:8]2[CH2:9][CH2:10][N:11]([CH2:12][C:13]([F:14])([F:15])[F:16])[CH2:17][CH2:18]2)[cH:19][cH:20]1
O=[N+]([O-])c1ccc(C2CCN(CC(F)(F)F)CC2)cc1
O=CNc1ccc(C2CCN(CC(F)(F)F)CC2)cc1
null
[Pd]
CCO.CCOC(=O)C
Functional Group Interconversion
OtherReaction
81e9c00cc56669b3382585c40a086ed7e5aaaab80bc5382ed121e4d5a293b433
013ea010a5fc8551154a976160b11b17bb85fae400bd37b37532ea17a3df22d8
c1ccc(C2CCNCC2)cc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[O;D1;H0:5]=[C:6]-[NH;D2;+0:1]-[c:2](:[c:3]):[c:4]
77.8
[{"value": 77.8, "product": "FC(CN1CCC(CC1)C1=CC=C(C=C1)NC=O)(F)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Ammonium formate (1.38 g, 22 mmol) and 10% Pd/C (230 mg, 0.2 mmol) are added to a solution of 1-(2,2,2-trifluoroethyl)-4-(4-nitrophenyl)piperidine (1.26 g, 4.4 mmol) in EtOH (10 mL) and EtOAc (10 mL). The suspension is heated at reflux for 24 hours, adding further portions of ammonium formate (2 g) after 4 h and 8 h. T...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Secondary amide
null
null
c1ccccc1.C1CC[NH]CC1
null
[Pd].CCO.CCOC(=O)C
null
null
O=[N+]([O-])c1ccc(C2CCN(CC(F)(F)F)CC2)cc1>[Pd].CCO.CCOC(=O)C>O=CNc1ccc(C2CCN(CC(F)(F)F)CC2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2a806c2c14d04eb1937fed9f0b30ef37
O=CNc1ccc(C2CCN(CC(F)(F)F)CC2)cc1>>Nc1ccc(C2CCN(CC(F)(F)F)CC2)cc1
FC(CN1CCC(CC1)C1=CC=C(C=C1)NC=O)(F)F.Cl>>FC(CN1CCC(CC1)C1=CC=C(C=C1)N)(F)F
O=C[NH:1][c:2]1[cH:3][cH:4][c:5]([CH:6]2[CH2:7][CH2:8][N:9]([CH2:10][C:11]([F:12])([F:13])[F:14])[CH2:15][CH2:16]2)[cH:17][cH:18]1>>[NH2:1][c:2]1[cH:3][cH:4][c:5]([CH:6]2[CH2:7][CH2:8][N:9]([CH2:10][C:11]([F:12])([F:13])[F:14])[CH2:15][CH2:16]2)[cH:17][cH:18]1
O=CNc1ccc(C2CCN(CC(F)(F)F)CC2)cc1
Nc1ccc(C2CCN(CC(F)(F)F)CC2)cc1
null
null
CO
Reduction
Reduction of primary amides to amines
755df58c254dea764fdda078ffd678ec540bba057c83683be04c253f1270ac7b
025f7cefe51e71668ad5d09fca32df168e9b538347403e4d5c1748073e538adc
c1ccc(C2CCNCC2)cc1
O=C-[NH;D2;+0:1]-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
A solution of the formamide in MeOH (20 mL) is stirred at rt and HCl (conc., 1 mL) is added. The deep purple solution is heated at reflux for 1 h, cooled and the MeOH is evaporated. The residue is stirred with water (20 mL) and NaHCO3 (sat. aq.) is added until bubbling ceases. The mixture is extracted with DCM (20 mL, ...
10.6084/m9.figshare.5104873.v1
null
Secondary amide
Primary amine
null
null
c1ccccc1.C1CC[NH]CC1
Other
CO
null
null
O=CNc1ccc(C2CCN(CC(F)(F)F)CC2)cc1>CO>Nc1ccc(C2CCN(CC(F)(F)F)CC2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c81a802209604c4eadda7d37f101c2c4
Brc1ncc(Br)n2ncnc12.Nc1ccc(OCCN2CCOCC2)cc1>>Brc1cnc(Nc2ccc(OCCN3CCOCC3)cc2)c2ncnn12
C(C)(C)N(C(C)C)CC.CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2.BrC1=CN=C(C=2N1N=CN2)Br.N1(CCOCC1)CCOC1=CC=C(C=C1)N>>BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)OCCN2CCOCC2
Br[c:5]1[n:4][cH:3][c:2]([Br:1])[n:26]2[c:22]1[n:23][cH:24][n:25]2.[NH2:6][c:7]1[cH:8][cH:9][c:10]([O:11][CH2:12][CH2:13][N:14]2[CH2:15][CH2:16][O:17][CH2:18][CH2:19]2)[cH:20][cH:21]1>>[Br:1][c:2]1[cH:3][n:4][c:5]([NH:6][c:7]2[cH:8][cH:9][c:10]([O:11][CH2:12][CH2:13][N:14]3[CH2:15][CH2:16][O:17][CH2:18][CH2:19]3)[cH:20...
Brc1ncc(Br)n2ncnc12.Nc1ccc(OCCN2CCOCC2)cc1
Brc1cnc(Nc2ccc(OCCN3CCOCC3)cc2)c2ncnn12
null
null
CC(C)O
Heteroatom Alkylation and Arylation
N-arylation (Buchwald-Hartwig/Ullmann-Goldberg)
aecfb0ede2c5d7901fea69101287828edf21f7a6e48b6ff83fe43de0688f1ef1
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1cn2ncnc2c(Nc2ccc(OCCN3CCOCC3)cc2)n1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:1.[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[c:12]:[c:11](-[NH;D2;+0:10]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:1):[c:13]
86.2
[{"value": 86.0, "product": "BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)OCCN2CCOCC2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 86.2, "product": "BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)OCCN2CCOCC2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
95
CELSIUS
8
HOUR
According to the procedure described for Compound 6, step 1, 5,8-dibromo-[1,2,4]triazolo[1,5-a]pyrazine (0.5 g, 1.799 mmol), 4-(2-morpholin-4-yl-ethoxy)-phenylamine (0.6 g, 4.5 mmol) and N,N-diisopropylethylamine (0.47 mL, 2.7 mmol) in 2-propanol (6 mL) are stirred at 95° C. overnight. After evaporation of the solvent ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1cn2ncnc2cn1
c1cn2ncnc2cn1
c1ccccc1.C1COCC[NH]1.c1cn2ncnc2cn1
HBr
CC(C)O
95
8
Brc1ncc(Br)n2ncnc12.Nc1ccc(OCCN2CCOCC2)cc1>CC(C)O>Brc1cnc(Nc2ccc(OCCN3CCOCC3)cc2)c2ncnn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1ce1195ef0cd43baac590902bcd96267
Brc1cnc(Nc2ccc(OCCN3CCOCC3)cc2)c2ncnn12.CC1(C)OB(c2ccc3c(c2)CNC3=O)OC1(C)C>>O=C1NCc2cc(-c3cnc(Nc4ccc(OCCN5CCOCC5)cc4)c4ncnn34)ccc21
CC1(OB(OC1(C)C)C=1C=C2CNC(C2=CC1)=O)C.CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2.C(=O)([O-])[O-].[Na+].[Na+].BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)OCCN2CCOCC2>>O1CCN(CC1)CCOC1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C3CNC(C3=CC1)=O)N=CN2
Br[c:8]1[cH:9][n:10][c:11]([NH:12][c:13]2[cH:14][cH:15][c:16]([O:17][CH2:18][CH2:19][N:20]3[CH2:21][CH2:22][O:23][CH2:24][CH2:25]3)[cH:26][cH:27]2)[c:28]2[n:29][cH:30][n:31][n:32]12.CC1(C)OB([c:7]2[cH:6][c:5]3[c:35]([cH:34][cH:33]2)[C:2](=[O:1])[NH:3][CH2:4]3)OC1(C)C>>[O:1]=[C:2]1[NH:3][CH2:4][c:5]2[cH:6][c:7](-[c:8]3[...
Brc1cnc(Nc2ccc(OCCN3CCOCC3)cc2)c2ncnn12.CC1(C)OB(c2ccc3c(c2)CNC3=O)OC1(C)C
O=C1NCc2cc(-c3cnc(Nc4ccc(OCCN5CCOCC5)cc4)c4ncnn34)ccc21
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O1CCOCC1
C-C Coupling
Suzuki coupling with boronic esters
0e514a9992c96da29f2ec2414679fb7906a3f635b15b1ade3e33600ae6778418
b42efb3b6a7742d5af594c6a3031e487327e58e9f8c2f428ee68996c98377910
O=C1NCc2cc(-c3cnc(Nc4ccc(OCCN5CCOCC5)cc4)c4ncnn34)ccc21
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1.C-C1(-C)-O-B(-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14])-O-C-1(-C)-C>>[c:12]:[c:11]:[c;H0;D3;+0:10](-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1):[c:13]:[c:14]
69
[{"value": 69.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound may be prepared using the methods as described for Compound 6, step 4, using (5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-yl)-[4-(2-morpholin-4-yl-ethoxy)-phenyl]-amine (80 mg, 0.19 mmol), 5-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-2,3-dihydro-isoindol-1-one (74 mg, 0.29 mmol), and Pd(PPh3)4 (55 mg, 0.0...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic ester
null
c1cn2ncnc2cn1.B1OCCO1.c1ccc2c(c1)CNC2
c1ccc2c(c1)CNC2.c1cn2ncnc2cn1
c1ccc2c(c1)CNC2.c1ccccc1.C1COCC[NH]1.c1cn2ncnc2cn1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1
null
null
Brc1cnc(Nc2ccc(OCCN3CCOCC3)cc2)c2ncnn12.CC1(C)OB(c2ccc3c(c2)CNC3=O)OC1(C)C>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1>O=C1NCc2cc(-c3cnc(Nc4ccc(OCCN5CCOCC5)cc4)c4ncnn34)ccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ac7bb6b97fb5453da4d1ade21276404c
Brc1ncc(Br)n2ncnc12.Nc1ccc(N2CCOCC2)cc1F>>Fc1cc(N2CCOCC2)ccc1Nc1ncc(Br)n2ncnc12
FC1=C(C=CC(=C1)N1CCOCC1)N.N12CCN(CC1)CC2.CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2.CCN(C(C)C)C(C)C.BrC1=CN=C(C=2N1N=CN2)Br>>BrC1=CN=C(C=2N1N=CN2)NC2=C(C=C(C=C2)N2CCOCC2)F
Br[c:15]1[n:16][cH:17][c:18]([Br:19])[n:20]2[n:21][cH:22][n:23][c:24]12.[F:1][c:2]1[cH:3][c:4]([N:5]2[CH2:6][CH2:7][O:8][CH2:9][CH2:10]2)[cH:11][cH:12][c:13]1[NH2:14]>>[F:1][c:2]1[cH:3][c:4]([N:5]2[CH2:6][CH2:7][O:8][CH2:9][CH2:10]2)[cH:11][cH:12][c:13]1[NH:14][c:15]1[n:16][cH:17][c:18]([Br:19])[n:20]2[n:21][cH:22][n:2...
Brc1ncc(Br)n2ncnc12.Nc1ccc(N2CCOCC2)cc1F
Fc1cc(N2CCOCC2)ccc1Nc1ncc(Br)n2ncnc12
null
null
CC(C)O
Heteroatom Alkylation and Arylation
N-arylation (Buchwald-Hartwig/Ullmann-Goldberg)
aecfb0ede2c5d7901fea69101287828edf21f7a6e48b6ff83fe43de0688f1ef1
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1cn2ncnc2c(Nc2ccc(N3CCOCC3)cc2)n1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:1.[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[c:12]:[c:11](-[NH;D2;+0:10]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:1):[c:13]
42
[{"value": 42.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound may be prepared using methods as described for Compound 6, step 1, using 5,8-dibromo-[1,2,4]triazolo[1,5-a]pyrazine (0.105 g, 0.89 mmol), 2-fluoro-4-morpholin-4-yl-phenylamine (93 mg, 0.474 mmol), DIPEA (0.123 mL, 0.706 mmol) and 1,4-diazabicyclo[2.2.2]octane (53 mg, 0.472 mmol) in 2-propanol (2 mL). The ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1cn2ncnc2cn1
c1cn2ncnc2cn1
c1ccccc1.C1COCC[NH]1.c1cn2ncnc2cn1
HBr
CC(C)O
null
null
Brc1ncc(Br)n2ncnc12.Nc1ccc(N2CCOCC2)cc1F>CC(C)O>Fc1cc(N2CCOCC2)ccc1Nc1ncc(Br)n2ncnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-49a52185ac7d47708e965d2dad590b46
CC1(C)OB(c2cn[nH]c2)OC1(C)C.Fc1cc(N2CCOCC2)ccc1Nc1ncc(Br)n2ncnc12>>Fc1cc(N2CCOCC2)ccc1Nc1ncc(-c2cn[nH]c2)n2ncnc12
C(=O)([O-])[O-].[Na+].[Na+].CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2.BrC1=CN=C(C=2N1N=CN2)NC2=C(C=C(C=C2)N2CCOCC2)F.CC1(OB(OC1(C)C)C=1C=NNC1)C>>FC1=C(C=CC(=C1)N1CCOCC1)NC=1C=2N(C(=CN1)C=1C=NNC1)N=CN2
CC1(C)OB([c:19]2[cH:20][n:21][nH:22][cH:23]2)OC1(C)C.Br[c:18]1[cH:17][n:16][c:15]([NH:14][c:13]2[c:2]([F:1])[cH:3][c:4]([N:5]3[CH2:6][CH2:7][O:8][CH2:9][CH2:10]3)[cH:11][cH:12]2)[c:28]2[n:24]1[n:25][cH:26][n:27]2>>[F:1][c:2]1[cH:3][c:4]([N:5]2[CH2:6][CH2:7][O:8][CH2:9][CH2:10]2)[cH:11][cH:12][c:13]1[NH:14][c:15]1[n:16]...
CC1(C)OB(c2cn[nH]c2)OC1(C)C.Fc1cc(N2CCOCC2)ccc1Nc1ncc(Br)n2ncnc12
Fc1cc(N2CCOCC2)ccc1Nc1ncc(-c2cn[nH]c2)n2ncnc12
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O1CCOCC1
C-C Coupling
Suzuki coupling with boronic esters
3b077e58a8068174133a7eecad35957570f9290725408c31a955826b02d2e470
b42efb3b6a7742d5af594c6a3031e487327e58e9f8c2f428ee68996c98377910
c1nc2c(Nc3ccc(N4CCOCC4)cc3)ncc(-c3cn[nH]c3)n2n1
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1.C-C1(-C)-O-B(-[c;H0;D3;+0:10]2:[c:11]:[#7;a:12]:[#7;a:13]:[c:14]:2)-O-C-1(-C)-C>>[#7;a:3]1:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:[c;H0;D3;+0:1](-[c;H0;D3;+0:10]2:[c:11]:[#7;a:12]:[#7;a:13]:[c:14]:2):[c:2]:1
38
[{"value": 38.0, "product": "FC1=C(C=CC(=C1)N1CCOCC1)NC=1C=2N(C(=CN1)C=1C=NNC1)N=CN2", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound may be prepared using methods as described for Compound 6, step 4, using (5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-yl)-(2-fluoro-4-morpholin-4-yl-phenyl)-amine (80 mg, 0.203 mmol), 4-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-1H-pyrazole (79 mg, 0.406 mmol), and Pd(PPh3)4 (59 mg, 0.051 mmol) in 1.5N Na...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic ester
null
B1OCCO1.c1cn[nH]c1.c1cn2ncnc2cn1
c1cn[nH]c1.c1cn2ncnc2cn1
c1ccccc1.C1COCC[NH]1.c1cn[nH]c1.c1cn2ncnc2cn1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1
null
null
CC1(C)OB(c2cn[nH]c2)OC1(C)C.Fc1cc(N2CCOCC2)ccc1Nc1ncc(Br)n2ncnc12>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1>Fc1cc(N2CCOCC2)ccc1Nc1ncc(-c2cn[nH]c2)n2ncnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0b97dc8358f6448f9d7204d6e5127b9c
CC(C)(C)[Si](C)(C)Cl.OCc1[nH]ncc1Br>>CC(C)(C)[SiH2]OC(C)(C)c1[nH]ncc1Br
C(C)OCC.BrC1=C(NN=C1)CO.[Si](C)(C)(C(C)(C)C)Cl.N1C=NC=C1>>BrC=1C=NNC1C(O[SiH2]C(C)(C)C)(C)C
Cl[Si:5]([C:2]([CH3:1])([CH3:3])[CH3:4])([CH3:8])[CH3:9].[OH:6][CH2:7][c:10]1[nH:11][n:12][cH:13][c:14]1[Br:15]>>[CH3:1][C:2]([CH3:3])([CH3:4])[SiH2:5][O:6][C:7]([CH3:8])([CH3:9])[c:10]1[nH:11][n:12][cH:13][c:14]1[Br:15]
CC(C)(C)[Si](C)(C)Cl.OCc1[nH]ncc1Br
CC(C)(C)[SiH2]OC(C)(C)c1[nH]ncc1Br
null
null
CN(C=O)C
C-C Coupling
OtherReaction
72a7646acc58c5670b83619272912c04ee14072de109d6c18abcc4d5ec13fed2
6b4e12c9a4ccedc8a11bbd8b74fb14ce3d1429a35cd9169d780ad652c7713b04
c1cn[nH]c1
Cl-[Si;H0;D4;+0:1](-[CH3;D1;+0:2])(-[CH3;D1;+0:3])-[C:4](-[C;D1;H3:5])(-[C;D1;H3:6])-[C;D1;H3:7].[OH;D1;+0:8]-[CH2;D2;+0:9]-[c:10]1:[#7;a:11]:[#7;a:12]:[c:13]:[c:14]:1>>[C;D1;H3:5]-[C:4](-[C;D1;H3:6])(-[C;D1;H3:7])-[SiH2;D2;+0:1]-[O;H0;D2;+0:8]-[C;H0;D4;+0:9](-[CH3;D1;+0:2])(-[CH3;D1;+0:3])-[c:10]1:[#7;a:11]:[#7;a:12]:...
98
[{"value": 98.0, "product": "BrC=1C=NNC1C(O[SiH2]C(C)(C)C)(C)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of (4-bromo-2H-pyrazol-3-yl)-methanol (0.64 mg, 3.63 mmol), tert-butyldimethylsilyl chloride (0.82 g, 5.45 mmol) and imidazole (0.42 g, 6.18 mmol) in N,N-dimethylformamide (20 mL) is stirred at room temperature overnight. The reaction mixture is diluted with a 50:50 mixture diethyl ether:ethyl acetate and wa...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Silyl protective group
null
null
null
c1cn[nH]c1
HCl
CN(C=O)C
null
null
CC(C)(C)[Si](C)(C)Cl.OCc1[nH]ncc1Br>CN(C=O)C>CC(C)(C)[SiH2]OC(C)(C)c1[nH]ncc1Br
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b51b16d24d9643aebecc23fbf8993b4b
C1=COCCC1.CC(C)(C)[SiH2]OC(C)(C)c1[nH]ncc1Br>>CC(C)(C)[SiH2]OC(C)(C)c1c(Br)cnn1C1CCCCO1.CC(C)(C)[SiH2]OC(C)(C)c1nn(C2CCCCO2)cc1Br
BrC=1C=NNC1C(O[SiH2]C(C)(C)C)(C)C.O1CCCC=C1.[H-].[Na+]>>BrC=1C(=NN(C1)C1OCCCC1)C(O[SiH2]C(C)(C)C)(C)C.BrC=1C=NN(C1C(O[SiH2]C(C)(C)C)(C)C)C1OCCCC1
[CH2:16]1[CH2:17][CH2:18][CH:19]=[CH:38][O:21]1.[CH3:1][C:2]([SiH2:5][O:6][C:7]([CH3:3])([c:10]1[c:11]([Br:12])[cH:13][n:14][nH:15]1)[CH3:23])([CH3:20])[CH3:36]>>[CH3:1][C:2]([CH3:3])([CH3:4])[SiH2:5][O:6][C:7]([CH3:8])([CH3:9])[c:10]1[c:11]([Br:12])[cH:13][n:14][n:15]1[CH:16]1[CH2:17][CH2:18][CH2:19][CH2:20][O:21]1.[C...
C1=COCCC1.CC(C)(C)[SiH2]OC(C)(C)c1[nH]ncc1Br
CC(C)(C)[SiH2]OC(C)(C)c1c(Br)cnn1C1CCCCO1.CC(C)(C)[SiH2]OC(C)(C)c1nn(C2CCCCO2)cc1Br
null
C(=O)(C(F)(F)F)O
null
Aromatic Heterocycle Formation
OtherReaction
88a97baded83eeb8083ea7731d7e5aac9e2c1855aabd5adda9923edfb9093a2e
b856992715d7b099e07bf70aa7d3c0c9c5967b1df181936fb26bd813f188f1b0
c1cnn(C2CCCCO2)c1.c1cnn(C2CCCCO2)c1
[C;D1;H3:1]-[C;H0;D4;+0:2](-[CH3;D1;+0:3])(-[CH3;D1;+0:4])-[#14:5]-[#8:6]-[C;H0;D4;+0:7](-[CH3;D1;+0:8])(-[CH3;D1;+0:9])-[c:10]1:[c:11]:[c:12]:[#7;a:13]:[nH;D2;+0:14]:1.[C:15]1-[C:16]-[CH;D2;+0:17]=[CH;D2;+0:18]-[O;H0;D2;+0:19]-[CH2;D2;+0:20]-1>>[#8:21]-[#14:22]-[C;H0;D4;+0:8](-[C;D1;H3:23])(-[C;D1;H3:24])-[C;D1;H3:25]...
111.8
[{"value": 56.0, "product": "BrC=1C=NN(C1C(O[SiH2]C(C)(C)C)(C)C)C1OCCCC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 111.8, "product": "BrC=1C=NN(C1C(O[SiH2]C(C)(C)C)(C)C)C1OCCCC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
90
CELSIUS
18
HOUR
4-Bromo-5-(tert-butyl-dimethyl-silanyloxymethyl)-1H-pyrazole (1 g, 3.45 mmol) is dissolved in 3,4-dihydro-2H-pyran (0.944 mL, 10.34 mmol) in the presence of a catalytic amount of TFA (0.0026 mL, 0.035 mmol). The reaction mixture is stirred at 90° C. for 18 hours, cooled and then quenched using NaH (4.69 mg, 0.206 mmol)...
10.6084/m9.figshare.5104873.v1
null
Ether
Aromatic halide.Ether.Ether
C1=COCCC1.c1cn[nH]c1
c1cn[nH]c1.C1CCOCC1.c1c[nH]nc1.C1CCOCC1
c1cn[nH]c1.C1CCOCC1.c1c[nH]nc1.C1CCOCC1
Other
C(=O)(C(F)(F)F)O
90
18
C1=COCCC1.CC(C)(C)[SiH2]OC(C)(C)c1[nH]ncc1Br>C(=O)(C(F)(F)F)O>CC(C)(C)[SiH2]OC(C)(C)c1c(Br)cnn1C1CCCCO1.CC(C)(C)[SiH2]OC(C)(C)c1nn(C2CCCCO2)cc1Br
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2603bbe820c04d83bd8522fba1cbcf86
CC(C)(C)[SiH2]OC(C)(C)c1c(-c2cnc(Nc3ccc(N4CCOCC4)cc3)c3ncnn23)cnn1C1CCCOC1>>OCc1[nH]ncc1-c1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12
C(C)(C)(C)[SiH2]OC(C1=NN(C=C1C1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2CCOCC2)C2COCCC2)(C)C.C(C)(C)(C)[SiH2]OC(C1=C(C=NN1C1COCCC1)C1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2CCOCC2)(C)C.Cl>>O1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=NNC1CO)N=CN2
CC(C)(C)[SiH2][O:1][C:2](C)(C)[c:3]1[n:4](C2CCCOC2)[n:5][cH:6][c:7]1-[c:8]1[cH:9][n:10][c:11]([NH:12][c:13]2[cH:14][cH:15][c:16]([N:17]3[CH2:18][CH2:19][O:20][CH2:21][CH2:22]3)[cH:23][cH:24]2)[c:25]2[n:26][cH:27][n:28][n:29]12>>[OH:1][CH2:2][c:3]1[nH:4][n:5][cH:6][c:7]1-[c:8]1[cH:9][n:10][c:11]([NH:12][c:13]2[cH:14][cH...
CC(C)(C)[SiH2]OC(C)(C)c1c(-c2cnc(Nc3ccc(N4CCOCC4)cc3)c3ncnn23)cnn1C1CCCOC1
OCc1[nH]ncc1-c1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12
null
null
CO
Reduction
OtherReaction
b83aaa72880f67296b021396a923e807e99ab3f7555f05c773f6f062a070e931
f3c13c34886a9ee39fc7fda8af9901946f6871b5562065675a15384eea5a8281
c1nc2c(Nc3ccc(N4CCOCC4)cc3)ncc(-c3cn[nH]c3)n2n1
C-C(-C)(-C)-[SiH2]-[O;H0;D2;+0:1]-[C;H0;D4;+0:2](-C)(-C)-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[n;H0;D3;+0:7]:1-C1-C-C-C-O-C-1>>[OH;D1;+0:1]-[CH2;D2;+0:2]-[c:3]1:[c:4]:[c:5]:[#7;a:6]:[nH;D2;+0:7]:1
null
[]
null
null
null
null
A solution of {5-[3-(tert-butyl-dimethyl-silanyloxymethyl)-1-(tetrahydro-pyran-3-yl)-1H-pyrazol-4-yl]-[1,2,4]triazolo[1,5-a]pyrazin-8-yl}-(4-morpholin-4-yl-phenyl)-amine and {5-[5-(tert-butyl-dimethyl-silanyloxymethyl)-1-(tetrahydro-pyran-3-yl)-1H-pyrazol-4-yl]-[1,2,4]triazolo[1,5-a]pyrazin-8-yl}-(4-morpholin-4-yl-phen...
10.6084/m9.figshare.5104873.v1
null
Ether
Primary alcohol
c1c[nH]nc1.C1CCOCC1
c1cn[nH]c1
c1cn[nH]c1.c1ccccc1.C1COCC[NH]1.c1cn2ncnc2cn1
HO-
CO
null
null
CC(C)(C)[SiH2]OC(C)(C)c1c(-c2cnc(Nc3ccc(N4CCOCC4)cc3)c3ncnn23)cnn1C1CCCOC1>CO>OCc1[nH]ncc1-c1cnc(Nc2ccc(N3CCOCC3)cc2)c2ncnn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5cf2e3e58a684a6fa54fbb1657752f1f
Brc1csc(Br)n1.CCOC(=O)OCC>>CCOC(=O)c1nc(Br)cs1
C(OCC)(OCC)=O.BrC=1N=C(SC1)Br.C(C)(C)[Mg]Cl>>C(C)OC(=O)C=1SC=C(N1)Br
Br[c:6]1[n:7][c:8]([Br:9])[cH:10][s:11]1.CCO[C:4]([O:3][CH2:2][CH3:1])=[O:5]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[n:7][c:8]([Br:9])[cH:10][s:11]1
Brc1csc(Br)n1.CCOC(=O)OCC
CCOC(=O)c1nc(Br)cs1
null
null
C1CCOC1
C-C Coupling
OtherReaction
eab4ec716edd47997f05b163a3ca9951e72a9d65e1083e2714b5da93c90a3eb8
bcd3559e95d57605d0e6e7a6ba9cc016318f006dee2eacb538f0c39f9d5391eb
c1cscn1
Br-[c;H0;D3;+0:1]1:[#16;a:2]:[c:3]:[c:4]:[#7;a:5]:1.C-C-O-[C;H0;D3;+0:6](=[O;D1;H0:7])-[#8:8]-[C:9]>>[C:9]-[#8:8]-[C;H0;D3;+0:6](=[O;D1;H0:7])-[c;H0;D3;+0:1]1:[#16;a:2]:[c:3]:[c:4]:[#7;a:5]:1
52
[{"value": 52.0, "product": "C(C)OC(=O)C=1SC=C(N1)Br", "details": "PERCENTYIELD", "is_desired": false}]
0
CELSIUS
0.25
HOUR
To a solution of dibromothiazole (1 g, 4.15 mmol) in THF (15 mL) at 0° C., is added dropwise a solution of iPrMgCl in THF (2 M, 2.3 mL, 4.57 mmol, 1.10 equiv.). The reaction is stirred at 0° C. for 0.25 h. To the resulting orange solution is added via a cannula, diethyl carbonate (3 mL) in THF (5 ml). The resulting gre...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Carbonic Ester
Ester
c1cscn1
c1cscn1
c1cscn1
HBr
C1CCOC1
0
0.25
Brc1csc(Br)n1.CCOC(=O)OCC>C1CCOC1>CCOC(=O)c1nc(Br)cs1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d3bbd687e934429f83c1107e159f79da
CCOC(=O)c1nc(Br)cs1.CN>>CNC(=O)c1nc(Br)cs1
C(C)OC(=O)C=1SC=C(N1)Br.CN>>CNC(=O)C=1SC=C(N1)Br
CCO[C:3](=[O:4])[c:5]1[n:6][c:7]([Br:8])[cH:9][s:10]1.[CH3:1][NH2:2]>>[CH3:1][NH:2][C:3](=[O:4])[c:5]1[n:6][c:7]([Br:8])[cH:9][s:10]1
CCOC(=O)c1nc(Br)cs1.CN
CNC(=O)c1nc(Br)cs1
null
null
CO
Acylation
Aminolysis of esters
04c54ce22aa9bc0cea0de3d900446bcab51cf02bebeb606fa788a47dcd0e37ff
4335147c9ad02004b7c12428d7eac0b2e7e0e2017adc471d01c387239de8017d
c1cscn1
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#16;a:4]:[c:5]:[c:6]:[#7;a:7]:1.[C;D1;H3:8]-[NH2;D1;+0:9]>>[C;D1;H3:8]-[NH;D2;+0:9]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#16;a:4]:[c:5]:[c:6]:[#7;a:7]:1
null
[]
null
null
8
HOUR
4-Bromothiazole-2-carboxylic acid ethyl ester (500 mg, 2.13 mmol) is dissolved in methanol (1 mL) and methyl amine in methanol (10 mL) is added. The mixture is stirred overnight at room temperature. Evaporation of the solvent under reduced pressure affords the title compound as yellow solid. LCMS: Rt 0.92 min (100%) m/...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine
Secondary amide
null
null
c1cscn1
HO-
CO
null
8
CCOC(=O)c1nc(Br)cs1.CN>CO>CNC(=O)c1nc(Br)cs1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6069cd44fe0e4069aeb6700cbe77f949
COC(=O)c1ccc(Br)cc1CBr.N>>O=C1NCc2cc(Br)ccc21
COC(C1=C(C=C(C=C1)Br)CBr)=O.N>>BrC=1C=C2CNC(C2=CC1)=O
CO[C:2](=[O:1])[c:11]1[c:5]([CH2:4]Br)[cH:6][c:7]([Br:8])[cH:9][cH:10]1.[NH3:3]>>[O:1]=[C:2]1[NH:3][CH2:4][c:5]2[cH:6][c:7]([Br:8])[cH:9][cH:10][c:11]21
COC(=O)c1ccc(Br)cc1CBr.N
O=C1NCc2cc(Br)ccc21
null
null
null
Acylation
OtherReaction
bfe20f0aa9f011cd97f8730d82b7c7716781d101d55a13d6080c38f132dfa20e
64fe73e2e83384d508c35f2187876b5b9badfa6118b2f44eff0dc89bfcf766e3
O=C1NCc2ccccc21
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4](-[C;H0;D3;+0:5](=[O;D1;H0:6])-O-C):[c:7].[NH3;D0;+0:8]>>[O;D1;H0:6]=[C;H0;D3;+0:5]1-[NH;D2;+0:8]-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]-1:[c:7]
65
[{"value": 65.0, "product": "BrC=1C=C2CNC(C2=CC1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
4-Bromo-2-bromomethyl-benzoic acid methyl ester (0.5 g, 16.2 mmol) is treated with methanolic ammonia (10 mL, 7 N NH3 in MeOH) for 5 minutes at 90° C. After cooling to room temperature a precipitate is formed, collected by filtration and washed with a small amount of methanol to afford the title compound as a colourles...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester
Secondary amide
null
c1ccc2c(c1)CNC2
c1ccc2c(c1)CNC2
HBr
null
null
null
COC(=O)c1ccc(Br)cc1CBr.N>>O=C1NCc2cc(Br)ccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5b08441a8fae42b5aa4c28a3eb8bc8dc
CC(C)N1CCNCC1.O=[N+]([O-])c1ccc(Cl)nc1>>CC(C)N1CCN(c2ccc([N+](=O)[O-])cn2)CC1
ClC1=NC=C(C=C1)[N+](=O)[O-].C(C)(C)N1CCNCC1.C(=O)([O-])[O-].[K+].[K+]>>C(C)(C)N1CCN(CC1)C1=NC=C(C=C1)[N+](=O)[O-]
[CH3:1][CH:2]([CH3:3])[N:4]1[CH2:5][CH2:6][NH:7][CH2:17][CH2:18]1.Cl[c:8]1[cH:9][cH:10][c:11]([N+:12](=[O:13])[O-:14])[cH:15][n:16]1>>[CH3:1][CH:2]([CH3:3])[N:4]1[CH2:5][CH2:6][N:7]([c:8]2[cH:9][cH:10][c:11]([N+:12](=[O:13])[O-:14])[cH:15][n:16]2)[CH2:17][CH2:18]1
CC(C)N1CCNCC1.O=[N+]([O-])c1ccc(Cl)nc1
CC(C)N1CCN(c2ccc([N+](=O)[O-])cn2)CC1
null
null
C1CCOC1
Heteroatom Alkylation and Arylation
Ullmann-Goldberg Substitution amine
fa523b05de53c4b0abc4cfee73617ebc93929b0985f4e85a4f5201b7c9df83f1
b6b8e2cdb45054a35f5e8157d624f852c0601a09401556706e166b19536eb7a7
c1ccc(N2CCNCC2)nc1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5].[#7:6]1-[C:7]-[C:8]-[NH;D2;+0:9]-[C:10]-[C:11]-1>>[c:5]:[c:4]:[c;H0;D3;+0:1](-[N;H0;D3;+0:9]1-[C:8]-[C:7]-[#7:6]-[C:11]-[C:10]-1):[#7;a:2]:[c:3]
null
[]
50
CELSIUS
4
HOUR
To a solution of 2-chloro-5-nitropyridine (2.5 g, 15.7 mmol) in THF (25 mL), are added 1-isopropylpiperazine (2.01 g, 15.7 mmol) and K2CO3 (3.25 g, 23.6 mmol). The reaction mixture is stirred at 50° C. for 4 hours and then at 70° C. overnight. The solvent is removed in vacuo and the resultant orange solid is triturated...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Secondary amine
Tertiary amine
C1C[NH]CCN1.c1ccncc1
C1C[NH]CC[NH]1.c1ccncc1
C1C[NH]CC[NH]1.c1ccncc1
HCl
C1CCOC1
50
4
CC(C)N1CCNCC1.O=[N+]([O-])c1ccc(Cl)nc1>C1CCOC1>CC(C)N1CCN(c2ccc([N+](=O)[O-])cn2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c30382f053ff4f0eb8c94e28cb95ba2f
CC(C)N1CCN(c2ccc([N+](=O)[O-])cn2)CC1>>CC(C)N1CCN(c2ccc(N)cn2)CC1
C(C)(C)N1CCN(CC1)C1=NC=C(C=C1)[N+](=O)[O-].O.O.[Sn](Cl)Cl.Cl>>C(C)(C)N1CCN(CC1)C1=CC=C(C=N1)N
O=[N+:12]([O-])[c:11]1[cH:10][cH:9][c:8]([N:7]2[CH2:6][CH2:5][N:4]([CH:2]([CH3:1])[CH3:3])[CH2:16][CH2:15]2)[n:14][cH:13]1>>[CH3:1][CH:2]([CH3:3])[N:4]1[CH2:5][CH2:6][N:7]([c:8]2[cH:9][cH:10][c:11]([NH2:12])[cH:13][n:14]2)[CH2:15][CH2:16]1
CC(C)N1CCN(c2ccc([N+](=O)[O-])cn2)CC1
CC(C)N1CCN(c2ccc(N)cn2)CC1
null
null
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc(N2CCNCC2)nc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]:[#7;a:5]:[c:6]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]:[#7;a:5]:[c:6]
86
[{"value": 86.0, "product": "C(C)(C)N1CCN(CC1)C1=CC=C(C=N1)N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 85.7, "product": "C(C)(C)N1CCN(CC1)C1=CC=C(C=N1)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
1-Isopropyl-4-(5-nitro-pyridin-2-yl)-piperazine (0.9 g, 3.6 mmol) is dissolved in MeOH (20 mL) and tin (II) dichloride dihydrate (4 g, 18 mmol) is added. The mixture is cooled using a water bath and conc. HCl is added (4 mL). The reaction is stirred at room temperature overnight. After removing the methanol, the result...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
C1C[NH]CC[NH]1.c1ccncc1
Other
CO
null
8
CC(C)N1CCN(c2ccc([N+](=O)[O-])cn2)CC1>CO>CC(C)N1CCN(c2ccc(N)cn2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-bd472570412c4388a8695015086d4763
CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cn2)CC1.CC1(C)OB(c2ccc3c(c2)CNC3=O)OC1(C)C>>CC(C)N1CCN(c2ccc(Nc3ncc(-c4ccc5c(c4)CNC5=O)n4ncnc34)cn2)CC1
CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2.BrC1=CN=C(C=2N1N=CN2)NC=2C=NC(=CC2)N2CCN(CC2)C(C)C.CC1(OB(OC1(C)C)C=1C=C2CNC(C2=CC1)=O)C>>C(C)(C)N1CCN(CC1)C1=CC=C(C=N1)NC=1C=2N(C(=CN1)C=1C=C3CNC(C3=CC1)=O)N=CN2
Br[c:16]1[cH:15][n:14][c:13]([NH:12][c:11]2[cH:10][cH:9][c:8]([N:7]3[CH2:6][CH2:5][N:4]([CH:2]([CH3:1])[CH3:3])[CH2:35][CH2:34]3)[n:33][cH:32]2)[c:31]2[n:27]1[n:28][cH:29][n:30]2.CC1(C)OB([c:17]2[cH:18][cH:19][c:20]3[c:21]([cH:22]2)[CH2:23][NH:24][C:25]3=[O:26])OC1(C)C>>[CH3:1][CH:2]([CH3:3])[N:4]1[CH2:5][CH2:6][N:7]([...
CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cn2)CC1.CC1(C)OB(c2ccc3c(c2)CNC3=O)OC1(C)C
CC(C)N1CCN(c2ccc(Nc3ncc(-c4ccc5c(c4)CNC5=O)n4ncnc34)cn2)CC1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O1CCOCC1.C(=O)([O-])[O-].[Na+].[Na+]
C-C Coupling
Suzuki coupling with boronic esters
0e514a9992c96da29f2ec2414679fb7906a3f635b15b1ade3e33600ae6778418
b42efb3b6a7742d5af594c6a3031e487327e58e9f8c2f428ee68996c98377910
O=C1NCc2cc(-c3cnc(Nc4ccc(N5CCNCC5)nc4)c4ncnn34)ccc21
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1.C-C1(-C)-O-B(-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14])-O-C-1(-C)-C>>[c:12]:[c:11]:[c;H0;D3;+0:10](-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1):[c:13]:[c:14]
null
[]
null
null
null
null
This compound may be prepared using methods as described for Compound 6, step 4, using 5-bromo-N-(6-(4-isopropylpiperazin-1-yl)pyridin-3-yl)-[1,2,4]triazolo[1,5-a]pyrazin-8-amine (50 mg, 0.12 mmol), 5-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-2,3-dihydro-isoindol-1-one (56 mg, 0.216 mmol) and Pd(PPh3)4 (35 mg, 0.0...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic ester
null
c1cn2ncnc2cn1.B1OCCO1.c1ccc2c(c1)CNC2
c1ccc2c(c1)CNC2.c1cn2ncnc2cn1
C1C[NH]CC[NH]1.c1ccncc1.c1ccc2c(c1)CNC2.c1cn2ncnc2cn1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1.C(=O)([O-])[O-].[Na+].[Na+]
null
null
CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cn2)CC1.CC1(C)OB(c2ccc3c(c2)CNC3=O)OC1(C)C>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1.C(=O)([O-])[O-].[Na+].[Na+]>CC(C)N1CCN(c2ccc(Nc3ncc(-c4ccc5c(...
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-724cebcaefc44d49bb6b890480f69a3c
CCOC(CBr)OCC.Sc1ccccc1Br>>CCOC=CSc1ccccc1Br
O.BrCC(OCC)OCC.BrC1=C(C=CC=C1)S.C([O-])([O-])=O.[K+].[K+]>>BrC1=C(C=CC=C1)SC=COCC
CCO[CH:4]([O:3][CH2:2][CH3:1])[CH2:5]Br.[SH:6][c:7]1[cH:8][cH:9][cH:10][cH:11][c:12]1[Br:13]>>[CH3:1][CH2:2][O:3][CH:4]=[CH:5][S:6][c:7]1[cH:8][cH:9][cH:10][cH:11][c:12]1[Br:13]
CCOC(CBr)OCC.Sc1ccccc1Br
CCOC=CSc1ccccc1Br
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
OtherReaction
a25c6e5ccd76fa864f6dd7ef671ee1eef69d64bf541b51af8438489add3390ca
bc651cc20acc61bf6e1ff09b340bd291b6db4e7662a32e932f07f0a8e438a76d
c1ccccc1
Br-[CH2;D2;+0:1]-[CH;D3;+0:2](-O-C-C)-[#8:3]-[C:4].[SH;D1;+0:5]-[c:6](:[c:7]):[c:8]>>[C:4]-[#8:3]-[CH;D2;+0:2]=[CH;D2;+0:1]-[S;H0;D2;+0:5]-[c:6](:[c:7]):[c:8]
null
[]
null
null
2
HOUR
To a solution of 2-bromothiophenol (10.50 g, 55.87 mmol) in dry DMF (50 mL) under nitrogen is added cautiously potassium carbonate (9.2 mL, 61.46 mmol, 1.10 equiv.). Once bubbling has subsided, 2-bromo-1,1-diethoxyethane (8.46 g, 61.46 mmol, 1.10 equiv.) is added to the mixture and stirred for 2 h at room temperature. ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ether.Ether.Aromatic thiol
Ether.Monosulfide
null
null
c1ccccc1
HBr
CN(C)C=O
null
2
CCOC(CBr)OCC.Sc1ccccc1Br>CN(C)C=O>CCOC=CSc1ccccc1Br
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-25bb78cf37ed41c68f9f83ba102f470d
CCOC=CSc1ccccc1Br>>Brc1cccc2ccsc12
BrC1=C(C=CC=C1)SC=COCC>>BrC1=CC=CC2=C1SC=C2
CCO[CH:7]=[CH:8][S:9][c:10]1[c:2]([Br:1])[cH:3][cH:4][cH:5][cH:6]1>>[Br:1][c:2]1[cH:3][cH:4][cH:5][c:6]2[cH:7][cH:8][s:9][c:10]12
CCOC=CSc1ccccc1Br
Brc1cccc2ccsc12
null
null
ClC1=CC=CC=C1
Aromatic Heterocycle Formation
OtherReaction
3b3a47e1a37723cb89ea18d12710cf7a4e1e15dc1cbc211627933afbf6616922
4b36a288ef2269f6b903f0d10e5fd047b6de50e118af8eebc52b54cdfe6597f4
c1ccc2sccc2c1
C-C-O-[CH;D2;+0:1]=[CH;D2;+0:2]-[S;H0;D2;+0:3]-[c:4](:[c:5]):[cH;D2;+0:6]:[c:7]:[c:8]>>[c:5]:[c:4]1:[s;H0;D2;+0:3]:[cH;D2;+0:2]:[cH;D2;+0:1]:[c;H0;D3;+0:6]:1:[c:7]:[c:8]
35
[{"value": 35.0, "product": "BrC1=CC=CC2=C1SC=C2", "details": "PERCENTYIELD", "is_desired": false}]
70
CELSIUS
null
null
1-Bromo-2-(2-ethoxyvinylsulfanyl)benzene is dissolved in chlorobenzene (50 mL) and the solution is heated to 70° C. PPA (10.5 mL) is then added carefully and the biphasic mixture is heated at 150° C. overnight. The resulting dark syrup is allowed to cool down and the supernatant solvent removed by pipette. Chlorobenzen...
10.6084/m9.figshare.5104873.v1
null
Ether.Monosulfide
null
c1ccccc1
c1ccc2sccc2c1
c1ccc2sccc2c1
HO-
ClC1=CC=CC=C1
70
null
CCOC=CSc1ccccc1Br>ClC1=CC=CC=C1>Brc1cccc2ccsc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8557a574f6614ac88eef6422d26425a2
Brc1cccc2ccsc12.CCOC(=O)OCC>>CCOC(=O)c1cccc2ccsc12
C(OCC)(OCC)=O.BrC1=CC=CC2=C1SC=C2.[Mg].[Cl-].[NH4+].[Mg]>>C(C)OC(=O)C1=CC=CC2=C1SC=C2
Br[c:6]1[cH:7][cH:8][cH:9][c:10]2[cH:11][cH:12][s:13][c:14]12.CCO[C:4]([O:3][CH2:2][CH3:1])=[O:5]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][cH:9][c:10]2[cH:11][cH:12][s:13][c:14]12
Brc1cccc2ccsc12.CCOC(=O)OCC
CCOC(=O)c1cccc2ccsc12
null
null
C1CCOC1
C-C Coupling
OtherReaction
1f5ef588d5d8a9fcdbeceb32da0c7a3570945b63c30fa4b3e818afd47f4f8213
bcd3559e95d57605d0e6e7a6ba9cc016318f006dee2eacb538f0c39f9d5391eb
c1ccc2sccc2c1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](:[c:5]):[#16;a:6]:[c:7].C-C-O-[C;H0;D3;+0:8](=[O;D1;H0:9])-[#8:10]-[C:11]>>[C:11]-[#8:10]-[C;H0;D3;+0:8](=[O;D1;H0:9])-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](:[c:5]):[#16;a:6]:[c:7]
71
[{"value": 71.0, "product": "C(C)OC(=O)C1=CC=CC2=C1SC=C2", "details": "PERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
7-bromobenzo[b]thiophene (500 mg, 2.36 mmol) is dissolved in dry THF (5.0 mL) under nitrogen. Magnesium turnings (530 mg, 2.83 mmol, 1.20 equiv.) are added and the resulting mixture is heated at reflux until dissolution of the magnesium has occurred. The resulting cloudy yellow solution is allowed to cool to rt and die...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Carbonic Ester
Ester
c1ccc2sccc2c1
c1ccc2sccc2c1
c1ccc2sccc2c1
HBr
C1CCOC1
null
1
Brc1cccc2ccsc12.CCOC(=O)OCC>C1CCOC1>CCOC(=O)c1cccc2ccsc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1dccd73d7787490ab03944c011c536cb
CCOC(=O)c1cccc2ccsc12>>O=C(O)c1cccc2ccsc12
C(C)OC(=O)C1=CC=CC2=C1SC=C2.[OH-].[Na+]>>S1C2=C(C=C1)C=CC=C2C(=O)O
CC[O:3][C:2](=[O:1])[c:4]1[cH:5][cH:6][cH:7][c:8]2[cH:9][cH:10][s:11][c:12]12>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][cH:7][c:8]2[cH:9][cH:10][s:11][c:12]12
CCOC(=O)c1cccc2ccsc12
O=C(O)c1cccc2ccsc12
null
null
O.CO
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc2sccc2c1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]:[#16;a:6]>>[#16;a:6]:[c:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
59
[{"value": 59.0, "product": "S1C2=C(C=C1)C=CC=C2C(=O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 5.9, "product": "S1C2=C(C=C1)C=CC=C2C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
To a solution of benzo[b]thiophene-7-carboxylic acid ethyl ester (1.0 g, 48 mmol) in methanol (10 mL) and water (10 mL) is added sodium hydroxide (5 g, excess). The solution is stirred at room temperature for 30 min; at which point all the ester has been consumed. The reaction mixture is adjusted to pH 1 by adding 6M H...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccc2sccc2c1
Other
O.CO
null
0.5
CCOC(=O)c1cccc2ccsc12>O.CO>O=C(O)c1cccc2ccsc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1e72ea23b8e744db9713ae2ea73eeea8
N.O=C(O)c1cccc2ccsc12>>NC(=O)c1cccc2ccsc12
C(=O)(O)[O-].[Na+].S(=O)(Cl)Cl.S1C2=C(C=C1)C=CC=C2C(=O)O.N>>S1C2=C(C=C1)C=CC=C2C(=O)N
[NH3:1].O[C:2](=[O:3])[c:4]1[cH:5][cH:6][cH:7][c:8]2[cH:9][cH:10][s:11][c:12]12>>[NH2:1][C:2](=[O:3])[c:4]1[cH:5][cH:6][cH:7][c:8]2[cH:9][cH:10][s:11][c:12]12
N.O=C(O)c1cccc2ccsc12
NC(=O)c1cccc2ccsc12
null
null
ClCCl.O.CN(C)C=O
Acylation
Carboxylic acid to amide conversion
1283aef55d7ee699f097a8e5267689198c76ba671644401547f902657820236d
cb0a71c3fb37a76e96fbd81aae6f95a28398a03d1ad2c8e877085e735efb98f1
c1ccc2sccc2c1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](:[c:6]):[#16;a:7]:[c:8].[NH3;D0;+0:9]>>[NH2;D1;+0:9]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](:[c:6]):[#16;a:7]:[c:8]
null
[]
null
null
1
HOUR
A solution of benzo[b]thiophene-7-carboxylic acid (505 mg, 2.84 mmol) in dichloromethane (10 mL) is stirred at rt and thionyl chloride (669 mg, 5.68 mmol, 2.0 equiv.) is added, followed by DMF (0.06 mL), causing gas evolution. The resulting solution is stirred at rt for 1 hour. Aqueous ammonia (10 mL) is then added cau...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Primary amide
null
null
c1ccc2sccc2c1
HO-
ClCCl.O.CN(C)C=O
null
1
N.O=C(O)c1cccc2ccsc12>ClCCl.O.CN(C)C=O>NC(=O)c1cccc2ccsc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2a836a09183040de83db5060b8063243
NC(=O)c1cccc2ccsc12.O=C1CCC(=O)N1Br>>NC(=O)c1cccc2c(Br)csc12
C(C)(=O)O.S1C2=C(C=C1)C=CC=C2C(=O)N.C1CC(=O)N(C1=O)Br>>BrC=1C2=C(SC1)C(=CC=C2)C(=O)N
[NH2:1][C:2](=[O:3])[c:4]1[cH:5][cH:6][cH:7][c:8]2[cH:9][cH:11][s:12][c:13]12.O=C1CCC(=O)N1[Br:10]>>[NH2:1][C:2](=[O:3])[c:4]1[cH:5][cH:6][cH:7][c:8]2[c:9]([Br:10])[cH:11][s:12][c:13]12
NC(=O)c1cccc2ccsc12.O=C1CCC(=O)N1Br
NC(=O)c1cccc2c(Br)csc12
null
null
ClCCl
Functional Group Interconversion
Bromination
e44d0870c7c18b28c8897b5e91cec6d880d9714f95f6ff4571946e55f765cc6c
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
c1ccc2sccc2c1
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[N;D1;H2:2]-[C:3](=[O;D1;H0:4])-[c:5]:[c:6]1:[#16;a:7]:[c:8]:[cH;D2;+0:9]:[c:10]:1:[c:11]>>[Br;H0;D1;+0:1]-[c;H0;D3;+0:9]1:[c:8]:[#16;a:7]:[c:6](:[c:5]-[C:3](-[N;D1;H2:2])=[O;D1;H0:4]):[c:10]:1:[c:11]
79
[{"value": 79.0, "product": "BrC=1C2=C(SC1)C(=CC=C2)C(=O)N", "details": "PERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
A solution of benzo[b]thiophene-7-carboxylic acid amide (500 mg, 2.82 mmol) in dichloromethane (5 mL) is stirred at rt and acetic acid (5 mL) is added followed by NBS (750 mg, 4.23 mmol, 1.5 equiv.). The reaction is stirred at room temperature for 1 hour at which point LC-MS analysis shows full conversion of the starti...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1ccc2sccc2c1.C1CCNC1
c1ccc2sccc2c1
c1ccc2sccc2c1
HO-
ClCCl
null
1
NC(=O)c1cccc2ccsc12.O=C1CCC(=O)N1Br>ClCCl>NC(=O)c1cccc2c(Br)csc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-28eca8fe9b3f4156b195ed7665d89339
Cc1cc(Br)ccn1>>Cc1cc(Br)cc[n+]1[O-]
BrC1=CC(=NC=C1)C.C1=CC(=CC(=C1)Cl)C(=O)OO>>BrC1=CC(=[N+](C=C1)[O-])C
[CH3:1][c:2]1[cH:3][c:4]([Br:5])[cH:6][cH:7][n:8]1>>[CH3:1][c:2]1[cH:3][c:4]([Br:5])[cH:6][cH:7][n+:8]1[O-:9]
Cc1cc(Br)ccn1
Cc1cc(Br)cc[n+]1[O-]
null
null
C(Cl)Cl
Functional Group Interconversion
OtherReaction
54415aed4bb61f76efee9ed140374352608210a9fed7c372975c12eb7023cea2
f1bbf9aa3c82f5e49be9f6d53533b6bb152f359232b6d32090c168949766aa71
c1cc[nH+]cc1
[C;D1;H3:1]-[c:2](:[c:3]):[n;H0;D2;+0:4]:[c:5]:[c:6]>>[C;D1;H3:1]-[c:2](:[c:3]):[n+;H0;D3:4](-[O;-;D1;H0:7]):[c:5]:[c:6]
null
[]
null
null
3
HOUR
A solution of 4-bromo-2-methylpyridine (5 g, 29 mmol) in DCM (20 mL) is cooled to 0° C. and m-CPBA (7.55 g, 43.87 mmol, 1.5 equiv.) is added portionwise over 30 min. The ice bath is then removed and the mixture is allowed to stir at room temperature for 3 hours. The resulting solution is diluted with sodium bicarbonate...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ccncc1
C1=CC=[NH+]C=C1
C1=CC=[NH+]C=C1
null
C(Cl)Cl
null
3
Cc1cc(Br)ccn1>C(Cl)Cl>Cc1cc(Br)cc[n+]1[O-]
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0c44e6b863894bd3bbec0160a1725659
CC(=O)OC(C)=O.Cc1cc(Br)cc[n+]1[O-]>>CC(=O)OCc1cc(Br)ccn1
BrC1=CC(=[N+](C=C1)[O-])C.C(C)(=O)OC(C)=O>>BrC1=CC(=NC=C1)COC(C)=O
CC(=O)[O:4][C:2]([CH3:1])=[O:3].[O-][n+:12]1[c:6]([CH3:5])[cH:7][c:8]([Br:9])[cH:10][cH:11]1>>[CH3:1][C:2](=[O:3])[O:4][CH2:5][c:6]1[cH:7][c:8]([Br:9])[cH:10][cH:11][n:12]1
CC(=O)OC(C)=O.Cc1cc(Br)cc[n+]1[O-]
CC(=O)OCc1cc(Br)ccn1
null
null
C(Cl)Cl
Protection
OtherReaction
f4e85b633bf4e79d1b81c036d2f4e246a93c2eb8ec0202f93c45d73e710e4f0d
dd0b9e5a615173b1d6c9fe991a352f69d24fef80f4bf0eeab7c46667d446dcd0
c1ccncc1
C-C(=O)-[O;H0;D2;+0:1]-[C:2](-[C;D1;H3:3])=[O;D1;H0:4].[CH3;D1;+0:5]-[c:6](:[c:7]):[n+;H0;D3:8](-[O-]):[c:9]:[c:10]>>[C;D1;H3:3]-[C:2](=[O;D1;H0:4])-[O;H0;D2;+0:1]-[CH2;D2;+0:5]-[c:6](:[c:7]):[n;H0;D2;+0:8]:[c:9]:[c:10]
null
[]
null
null
1
HOUR
To a solution of 4-bromo-2-methylpyridine-1-oxide (4.00 g, 21.40 mmol) in DCM (20 mL) is added acetic anhydride (6 mL). The mixture is stirred at room temperature for 1 hour and then heated at reflux overnight. The solvent is removed under vacuum and the crude product is filtered through a silica plug, eluting with DCM...
10.6084/m9.figshare.5104873.v1
null
Anhydride
Ester
C1=CC=[NH+]C=C1
c1ccncc1
c1ccncc1
HO-
C(Cl)Cl
null
1
CC(=O)OC(C)=O.Cc1cc(Br)cc[n+]1[O-]>C(Cl)Cl>CC(=O)OCc1cc(Br)ccn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-fe5a3b077fb944c992dad3b05162cbbe
CC(=O)OCc1cc(B2OC(C)(C)C(C)(C)O2)ccn1.CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)CC1>>CC(=O)OCc1cc(-c2cnc(Nc3ccc(N4CCN(C(C)C)CC4)cc3)c3ncnn23)ccn1
BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2CCN(CC2)C(C)C.C([O-])([O-])=O.[K+].[K+].CC1(OB(OC1(C)C)C1=CC(=NC=C1)COC(C)=O)C>>C(C)(C)N1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C1=CC(=NC=C1)COC(C)=O)N=CN2
CC1(C)OB([c:8]2[cH:7][c:6]([CH2:5][O:4][C:2]([CH3:1])=[O:3])[n:36][cH:35][cH:34]2)OC1(C)C.Br[c:9]1[cH:10][n:11][c:12]([NH:13][c:14]2[cH:15][cH:16][c:17]([N:18]3[CH2:19][CH2:20][N:21]([CH:22]([CH3:23])[CH3:24])[CH2:25][CH2:26]3)[cH:27][cH:28]2)[c:29]2[n:30][cH:31][n:32][n:33]12>>[CH3:1][C:2](=[O:3])[O:4][CH2:5][c:6]1[cH...
CC(=O)OCc1cc(B2OC(C)(C)C(C)(C)O2)ccn1.CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)CC1
CC(=O)OCc1cc(-c2cnc(Nc3ccc(N4CCN(C(C)C)CC4)cc3)c3ncnn23)ccn1
null
C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.Cl[Pd]Cl.[Fe+2]
O1CCOCC1.O
C-C Coupling
Suzuki coupling with boronic esters
08de20b28f3001ce42d0191b8d9e5679e0920ef2236528a84beaa5bda4d8d3e0
b42efb3b6a7742d5af594c6a3031e487327e58e9f8c2f428ee68996c98377910
c1cc(-c2cnc(Nc3ccc(N4CCNCC4)cc3)c3ncnn23)ccn1
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1.C-C1(-C)-O-B(-[c;H0;D3;+0:10]2:[c:11]:[c:12]:[#7;a:13]:[c:14](-[C:15]):[c:16]:2)-O-C-1(-C)-C>>[C:15]-[c:14]1:[#7;a:13]:[c:12]:[c:11]:[c;H0;D3;+0:10](-[c;H0;D3;+0:1]2:[c:2]:[#7;a:3]:[c:4]:[c:5]3:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:3:2):[c:1...
null
[]
null
null
null
null
A suspension of (5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-yl)-[4-(4-isopropyl-piperazin-1-yl)phenyl]amine (300 mg, 0.723 mmol) and Pd(dppf)Cl2 (59 mg, 10 mol %) in 4/1 dioxane/water (5 mL) is stirred at rt and potassium carbonate (200 mg, 1.45 mmol, 2.0 equiv.) and acetic acid 4-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic ester
null
B1OCCO1.c1ccncc1.c1cn2ncnc2cn1
c1ccncc1.c1cn2ncnc2cn1
c1ccncc1.c1ccccc1.C1C[NH]CC[NH]1.c1cn2ncnc2cn1
HBr.B
C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.Cl[Pd]Cl.[Fe+2].O1CCOCC1.O
null
null
CC(=O)OCc1cc(B2OC(C)(C)C(C)(C)O2)ccn1.CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)CC1>C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.Cl[Pd]Cl.[Fe+2].O1CCOCC1.O>CC(=O)OCc1cc(-c2cnc(Nc3ccc(N4CCN(C(C)C)CC4)cc3)c3ncnn23)ccn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-45edd5e34d214dc19202bd9f88e1479c
CC(=O)OCc1cc(-c2cnc(Nc3ccc(N4CCN(C(C)C)CC4)cc3)c3ncnn23)ccn1>>CC(C)N1CCN(c2ccc(Nc3ncc(-c4ccnc(CO)c4)n4ncnc34)cc2)CC1
C(CC(O)(C(=O)O)CC(=O)O)(=O)O.C(C)(C)N1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C1=CC(=NC=C1)COC(C)=O)N=CN2.C([O-])([O-])=O.[K+].[K+]>>C(C)(C)N1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C1=CC(=NC=C1)CO)N=CN2
CC(=O)[O:23][CH2:22][c:21]1[n:20][cH:19][cH:18][c:17](-[c:16]2[cH:15][n:14][c:13]([NH:12][c:11]3[cH:10][cH:9][c:8]([N:7]4[CH2:6][CH2:5][N:4]([CH:2]([CH3:1])[CH3:3])[CH2:33][CH2:32]4)[cH:31][cH:30]3)[c:29]3[n:25]2[n:26][cH:27][n:28]3)[cH:24]1>>[CH3:1][CH:2]([CH3:3])[N:4]1[CH2:5][CH2:6][N:7]([c:8]2[cH:9][cH:10][c:11]([NH...
CC(=O)OCc1cc(-c2cnc(Nc3ccc(N4CCN(C(C)C)CC4)cc3)c3ncnn23)ccn1
CC(C)N1CCN(c2ccc(Nc3ncc(-c4ccnc(CO)c4)n4ncnc34)cc2)CC1
null
null
CO
Reduction
Hydrolysis or Hydrogenolysis of Carboxylic Esters or Thioesters
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
c1cc(-c2cnc(Nc3ccc(N4CCNCC4)cc3)c3ncnn23)ccn1
C-C(=O)-[O;H0;D2;+0:1]-[C:2]-[c:3]:[#7;a:4]>>[#7;a:4]:[c:3]-[C:2]-[OH;D1;+0:1]
12.5
[{"value": 12.5, "product": "C(C)(C)N1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C1=CC(=NC=C1)CO)N=CN2", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
Acetic acid 4-{8-[4-(4-isopropylpiperazin-1-yl)phenylamino]-[1,2,4]triazolo[1,5-a]pyrazin-5-yl}pyridin-2-ylmethyl ester is stirred at room temperature overnight in 10 mL of a 1.5 M solution of potassium carbonate in methanol. The pH is then brought to neutral by addition of 10% aqueous citric acid and the mixture is ex...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
C1C[NH]CC[NH]1.c1ccccc1.c1ccncc1.c1cn2ncnc2cn1
HO-
CO
null
null
CC(=O)OCc1cc(-c2cnc(Nc3ccc(N4CCN(C(C)C)CC4)cc3)c3ncnn23)ccn1>CO>CC(C)N1CCN(c2ccc(Nc3ncc(-c4ccnc(CO)c4)n4ncnc34)cc2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e652935c29cc4a9a9e672a5a24d1ecaa
CC(C)N1CCNCC1.O=[N+]([O-])c1ccc(F)cc1>>CC(C)N1CCN(c2ccc([N+](=O)[O-])cc2)CC1.N
FC1=CC=C(C=C1)[N+](=O)[O-].C(C)(C)N1CCNCC1.C(=O)([O-])[O-].[K+].[K+]>>N.C(C)(C)N1CCN(CC1)C1=CC=C(C=C1)[N+](=O)[O-]
[CH3:1][CH:2]([CH3:3])[N:4]1[CH2:5][CH2:6][NH:7][CH2:17][CH2:18]1.F[c:8]1[cH:9][cH:10][c:11]([N+:12](=[O:13])[O-:14])[cH:15][cH:16]1>>[CH3:1][CH:2]([CH3:3])[N:4]1[CH2:5][CH2:6][N:7]([c:8]2[cH:9][cH:10][c:11]([N+:12](=[O:13])[O-:14])[cH:15][cH:16]2)[CH2:17][CH2:18]1.[NH3:19]
CC(C)N1CCNCC1.O=[N+]([O-])c1ccc(F)cc1
CC(C)N1CCN(c2ccc([N+](=O)[O-])cc2)CC1.N
null
null
C1CCOC1
Functional Group Interconversion
Buchwald-Hartwig/Ullmann-Goldberg/N-arylation secondary amine
c6c38d29142a1aca5d86f02d4b0c2562460ca1aec33aa213f11cd4062c6e7363
39ece5c8e1ec3e350cfadd8e37bb010493b934313e1cd5367f16de670d62b5af
c1ccc(N2CCNCC2)cc1
F-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[#7:6]1-[C:7]-[C:8]-[NH;D2;+0:9]-[C:10]-[C:11]-1>>[c:5]:[c:4]:[c;H0;D3;+0:1](-[N;H0;D3;+0:9]1-[C:8]-[C:7]-[#7:6]-[C:11]-[C:10]-1):[c:2]:[c:3]
185.8
[{"value": 94.0, "product": "C(C)(C)N1CCN(CC1)C1=CC=C(C=C1)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 185.8, "product": "C(C)(C)N1CCN(CC1)C1=CC=C(C=C1)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To a solution of 4-fluoronitrobenzene (5 g, 35.4 mmol) in THF (50 mL), 1-isopropylpiperazine (4.54 g, 35.4 mmol) and K2CO3 (7.35 g, 53.2 mmol) are added. The reaction mixture is stirred at room temperature overnight. The solvent is removed in vacuo and the residue is partitioned between EtOAc and water. The organic lay...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Secondary amine
Tertiary amine
C1C[NH]CCN1.c1ccccc1
C1C[NH]CC[NH]1.c1ccccc1
C1C[NH]CC[NH]1.c1ccccc1
null
C1CCOC1
null
8
CC(C)N1CCNCC1.O=[N+]([O-])c1ccc(F)cc1>C1CCOC1>CC(C)N1CCN(c2ccc([N+](=O)[O-])cc2)CC1.N
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0b4e96c71ba444429a7116839d07adb3
CC(C)N1CCN(c2ccc([N+](=O)[O-])cc2)CC1>>CC(C)N1CCN(c2ccc(N)cc2)CC1
C(C)(C)N1CCN(CC1)C1=CC=C(C=C1)[N+](=O)[O-].O.O.[Sn](Cl)Cl.Cl>>C(C)(C)N1CCN(CC1)C1=CC=C(C=C1)N
O=[N+:12]([O-])[c:11]1[cH:10][cH:9][c:8]([N:7]2[CH2:6][CH2:5][N:4]([CH:2]([CH3:1])[CH3:3])[CH2:16][CH2:15]2)[cH:14][cH:13]1>>[CH3:1][CH:2]([CH3:3])[N:4]1[CH2:5][CH2:6][N:7]([c:8]2[cH:9][cH:10][c:11]([NH2:12])[cH:13][cH:14]2)[CH2:15][CH2:16]1
CC(C)N1CCN(c2ccc([N+](=O)[O-])cc2)CC1
CC(C)N1CCN(c2ccc(N)cc2)CC1
null
null
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc(N2CCNCC2)cc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
88
[{"value": 88.0, "product": "C(C)(C)N1CCN(CC1)C1=CC=C(C=C1)N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 87.9, "product": "C(C)(C)N1CCN(CC1)C1=CC=C(C=C1)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
1-Isopropyl-4-(4-nitro-phenyl)-piperazine (8.3 g, 33.2 mmol) is dissolved in MeOH (120 mL) and tin (II) dichloride dihydrate (37.4 g, 0.165 mol) is added. The mixture is cooled using a water bath and conc. HCl is added (36 mL). The reaction is stirred at room temperature overnight. After removing the methanol, the resu...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
C1C[NH]CC[NH]1.c1ccccc1
Other
CO
null
8
CC(C)N1CCN(c2ccc([N+](=O)[O-])cc2)CC1>CO>CC(C)N1CCN(c2ccc(N)cc2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2451d9c658d64830b9e953833027103d
Brc1ncc(Br)n2ncnc12.CC(C)N1CCN(c2ccc(N)cc2)CC1>>CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)CC1
C(C)(C)N(C(C)C)CC.BrC1=CN=C(C=2N1N=CN2)Br.CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2.C(C)(C)N1CCN(CC1)C1=CC=C(C=C1)N>>BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2CCN(CC2)C(C)C
Br[c:13]1[n:14][cH:15][c:16]([Br:17])[n:18]2[n:19][cH:20][n:21][c:22]12.[CH3:1][CH:2]([CH3:3])[N:4]1[CH2:5][CH2:6][N:7]([c:8]2[cH:9][cH:10][c:11]([NH2:12])[cH:23][cH:24]2)[CH2:25][CH2:26]1>>[CH3:1][CH:2]([CH3:3])[N:4]1[CH2:5][CH2:6][N:7]([c:8]2[cH:9][cH:10][c:11]([NH:12][c:13]3[n:14][cH:15][c:16]([Br:17])[n:18]4[n:19][...
Brc1ncc(Br)n2ncnc12.CC(C)N1CCN(c2ccc(N)cc2)CC1
CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)CC1
null
null
CC(C)O.C(C)OCC
Heteroatom Alkylation and Arylation
N-arylation (Buchwald-Hartwig/Ullmann-Goldberg)
aecfb0ede2c5d7901fea69101287828edf21f7a6e48b6ff83fe43de0688f1ef1
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1cn2ncnc2c(Nc2ccc(N3CCNCC3)cc2)n1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:1.[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[c:12]:[c:11](-[NH;D2;+0:10]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:1):[c:13]
null
[]
95
CELSIUS
8
HOUR
This compound may be prepared using methods as described for Compound 6, step 1, using 5,8-dibromo-[1,2,4]triazolo[1,5-a]pyrazine (2 g, 7.20 mmol), 4-(4-isopropyl-piperazin-1-yl)-phenylamine (1.89 g, 8.62 mmol) and N,N-diisopropylethylamine (1.88 mL, 10.8 mmol) in 2-propanol (30 mL) are stirred at 95° C. overnight. The...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1cn2ncnc2cn1
c1cn2ncnc2cn1
C1C[NH]CC[NH]1.c1ccccc1.c1cn2ncnc2cn1
HBr
CC(C)O.C(C)OCC
95
8
Brc1ncc(Br)n2ncnc12.CC(C)N1CCN(c2ccc(N)cc2)CC1>CC(C)O.C(C)OCC>CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2bd9f6e839c04a6b81426dc4856243ba
CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cn2)CC1.CC1(C)OB(c2coc(C(N)=O)c2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1>>CC(C)N1CCN(c2ccc(Nc3ncc(-c4coc(C(N)=O)c4)n4ncnc34)cc2)CC1
C(=O)([O-])[O-].[Na+].[Na+].CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2.BrC1=CN=C(C=2N1N=CN2)NC=2C=NC(=CC2)N2CCN(CC2)C(C)C.CC1(OB(OC1(C)C)C=1C=C(OC1)C(=O)N)C>>C(C)(C)N1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(OC1)C(=O)N)N=CN2
Br[c:16]1[cH:15][n:14][c:13]([NH:12][c:11]2[cH:10][cH:9][c:8]([N:7]3[CH2:6][CH2:5][N:4]([CH:2]([CH3:1])[CH3:3])[CH2:33][CH2:32]3)n[cH:30]2)[c:29]2[n:25]1[n:26][cH:27][n:28]2.CC1(C)OB([c:17]2[cH:18][o:19][c:20]([C:21]([NH2:22])=[O:23])[cH:24]2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)c[cH:31]2)CC1>>[CH3:1][...
CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cn2)CC1.CC1(C)OB(c2coc(C(N)=O)c2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1
CC(C)N1CCN(c2ccc(Nc3ncc(-c4coc(C(N)=O)c4)n4ncnc34)cc2)CC1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O1CCOCC1
C-C Coupling
OtherReaction
bf6d5b28da7df61f8a2a600f966a0396dfa36c38592da56b1b64fe7f4f86e80c
96e5f3628c1bd4659dd3e9821904115decf673d0e8e42bb7900b7f521b084c51
c1nc2c(Nc3ccc(N4CCNCC4)cc3)ncc(-c3ccoc3)n2n1
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4](-[#7:5]-[c:6]2:[c:7]:[c:8]:[c;H0;D3;+0:9](-[#7:10](-[C:11])-[C:12]):n:[cH;D2;+0:13]:2):[c:14]2:[#7;a:15]:[c:16]:[#7;a:17]:[#7;a:18]:2:1.C-C1(-C)-O-B(-[c;H0;D3;+0:19]2:[c:20]:[#8;a:21]:[c:22](-[C:23](-[N;D1;H2:24])=[O;D1;H0:25]):[c:26]:2)-O-C-1(-C)-C.C-N1-C-C-N(-c2:[cH;D2;+0:27]:c...
null
[]
null
null
null
null
This compound may be prepared using methods as described for Compound 6, step 4, using 5-bromo-N-(6-(4-isopropylpiperazin-1-yl)pyridin-3-yl)-[1,2,4]triazolo[1,5-a]pyrazin-8-amine (80 mg, 0.21 mmol), 4-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-furan-2-carboxylic acid amide (101 mg, 0.42 mmol), and Pd(PPh3)4 (62 mg,...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amide.Secondary amine.Tertiary amine.Tertiary amine.Boronic ester
null
c1ccncc1.c1cn2ncnc2cn1.B1OCCO1.c1ccoc1.C1CNCCN1.c1ccccc1.c1ccsc1.c1cn2ncnc2cn1
c1ccccc1.c1ccoc1.c1cn2ncnc2cn1
C1C[NH]CC[NH]1.c1ccccc1.c1ccoc1.c1cn2ncnc2cn1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1
null
null
CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cn2)CC1.CC1(C)OB(c2coc(C(N)=O)c2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1>CC(C)N1CC...
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9d1c0d6110ae46b5bac3913ab9dccf45
CC(C)N1CCN(c2ccc(Nc3ncc(-c4ccnc(CO)c4)n4ncnc34)cc2)CC1.CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cn2)CC1>>CC(C)N1CCN(c2ccc(Nc3ncc(-c4ccnc(CO)c4)n4ncnc34)cn2)CC1
C(C)(C)N1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C1=CC(=NC=C1)CO)N=CN2.BrC1=CN=C(C=2N1N=CN2)NC=2C=NC(=CC2)N2CCN(CC2)C(C)C>>C(C)(C)N1CCN(CC1)C1=CC=C(C=N1)NC=1C=2N(C(=CN1)C1=CC(=NC=C1)CO)N=CN2
CC(C)N1CCN(c2ccc(N[c:13]3[n:14][cH:15][c:16](-[c:17]4[cH:18][cH:19][n:20][c:21]([CH2:22][OH:23])[cH:24]4)[n:25]4[n:26][cH:27][n:28][c:29]34)cc2)CC1.Brc1cnc([NH:12][c:11]2[cH:10][cH:9][c:8]([N:7]3[CH2:6][CH2:5][N:4]([CH:2]([CH3:1])[CH3:3])[CH2:33][CH2:32]3)[n:31][cH:30]2)c2ncnn12>>[CH3:1][CH:2]([CH3:3])[N:4]1[CH2:5][CH2...
CC(C)N1CCN(c2ccc(Nc3ncc(-c4ccnc(CO)c4)n4ncnc34)cc2)CC1.CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cn2)CC1
CC(C)N1CCN(c2ccc(Nc3ncc(-c4ccnc(CO)c4)n4ncnc34)cn2)CC1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
d1da154872dac0258a7b32b30ccf643eba379743c3f0dca8db1ce5b9f2f57fb1
7d31f47e5761ed6e1805ce0becec02c3b3cb1ec75262e81cbdbb96933cfa3652
c1cc(-c2cnc(Nc3ccc(N4CCNCC4)nc3)c3ncnn23)ccn1
Br-c1:c:n:c(-[NH;D2;+0:1]-[c:2](:[c:3]):[c:4]:[#7;a:5]:[c:6]):c2:n:c:n:n:1:2.C-C(-C)-N1-C-C-N(-c2:c:c:c(-N-[c;H0;D3;+0:7]3:[#7;a:8]:[c:9]:[c:10]:[#7;a:11]4:[#7;a:12]:[c:13]:[#7;a:14]:[c:15]:4:3):c:c:2)-C-C-1>>[c:3]:[c:2](-[NH;D2;+0:1]-[c;H0;D3;+0:7]1:[#7;a:8]:[c:9]:[c:10]:[#7;a:11]2:[#7;a:12]:[c:13]:[#7;a:14]:[c:15]:2:...
null
[]
null
null
null
null
This compound may be prepared using the methods as described for Compound 83, using (5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-yl)-[6-(4-isopropylpiperazin-1-yl)pyridin-3-yl]amine in Step 4. LCMS: Rt=0.71 min (95%), m/z (ESI) 446 (M+H)+. Conditions: See reaction.notes.procedure_details. Workup: This compound may be prepa...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Secondary amine.Secondary amine.Tertiary amine.Tertiary amine
Secondary amine
C1CNCCN1.c1ccccc1.c1cn2ncnc2cn1.c1cn2ncnc2cn1
c1cn2ncnc2cn1
C1C[NH]CC[NH]1.c1ccncc1.c1ccncc1.c1cn2ncnc2cn1
HBr
null
null
null
CC(C)N1CCN(c2ccc(Nc3ncc(-c4ccnc(CO)c4)n4ncnc34)cc2)CC1.CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cn2)CC1>>CC(C)N1CCN(c2ccc(Nc3ncc(-c4ccnc(CO)c4)n4ncnc34)cn2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-66a7e911dae54a91aadb01fdc0782deb
CC(C)I.O=[N+]([O-])c1ccc(C2CCNCC2)cc1>>CC(C)N1CCC(c2ccc([N+](=O)[O-])cc2)CC1
[N+](=O)([O-])C1=CC=C(C=C1)C1CCNCC1.C(=O)([O-])[O-].[K+].[K+].IC(C)C>>C(C)(C)N1CCC(CC1)C1=CC=C(C=C1)[N+](=O)[O-]
I[CH:2]([CH3:1])[CH3:3].[NH:4]1[CH2:5][CH2:6][CH:7]([c:8]2[cH:9][cH:10][c:11]([N+:12](=[O:13])[O-:14])[cH:15][cH:16]2)[CH2:17][CH2:18]1>>[CH3:1][CH:2]([CH3:3])[N:4]1[CH2:5][CH2:6][CH:7]([c:8]2[cH:9][cH:10][c:11]([N+:12](=[O:13])[O-:14])[cH:15][cH:16]2)[CH2:17][CH2:18]1
CC(C)I.O=[N+]([O-])c1ccc(C2CCNCC2)cc1
CC(C)N1CCC(c2ccc([N+](=O)[O-])cc2)CC1
null
null
C(C)#N
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
e607f8be86144f88f0e003ba760672ae287bda7930358cc9b18df3f78aaa9c0b
fb63ba09935e18320be03869002f6d5d0f0321fe7dbcd94a5ae956c3effd182d
c1ccc(C2CCNCC2)cc1
I-[CH;D3;+0:1](-[C;D1;H3:2])-[C;D1;H3:3].[C:4]-[C:5]-[NH;D2;+0:6]-[C:7]-[C:8]>>[C:4]-[C:5]-[N;H0;D3;+0:6](-[CH;D3;+0:1](-[C;D1;H3:2])-[C;D1;H3:3])-[C:7]-[C:8]
99.8
[{"value": 99.8, "product": "C(C)(C)N1CCC(CC1)C1=CC=C(C=C1)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
4-(4-Nitrophenyl)piperidine (250 mg, 1.21 mmol), K2CO3 (170 mg, 1.21 mmol) and 2-iodopropane (240 μL, 2.4 mmol) are stirred in acetonitrile (3 mL) in a sealed tube at 120° C. for 45 min. The mixture is cooled and the solvent removed under reduced pressure. The residue is partitioned between DCM (20 mL) and water (5 mL)...
10.6084/m9.figshare.5104873.v1
null
Secondary halide.Secondary amine
Tertiary amine
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1.c1ccccc1
HI
C(C)#N
null
null
CC(C)I.O=[N+]([O-])c1ccc(C2CCNCC2)cc1>C(C)#N>CC(C)N1CCC(c2ccc([N+](=O)[O-])cc2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-47beca92f7bf46d2831f9c086d6c8527
CC(C)N1CCC(c2ccc([N+](=O)[O-])cc2)CC1>>CC(C)N1CCC(c2ccc(N)cc2)CC1
NN.C(C)(C)N1CCC(CC1)C1=CC=C(C=C1)[N+](=O)[O-]>>C(C)(C)N1CCC(CC1)C1=CC=C(C=C1)N
O=[N+:12]([O-])[c:11]1[cH:10][cH:9][c:8]([CH:7]2[CH2:6][CH2:5][N:4]([CH:2]([CH3:1])[CH3:3])[CH2:16][CH2:15]2)[cH:14][cH:13]1>>[CH3:1][CH:2]([CH3:3])[N:4]1[CH2:5][CH2:6][CH:7]([c:8]2[cH:9][cH:10][c:11]([NH2:12])[cH:13][cH:14]2)[CH2:15][CH2:16]1
CC(C)N1CCC(c2ccc([N+](=O)[O-])cc2)CC1
CC(C)N1CCC(c2ccc(N)cc2)CC1
null
[Pd]
CCO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc(C2CCNCC2)cc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
72.2
[{"value": 72.2, "product": "C(C)(C)N1CCC(CC1)C1=CC=C(C=C1)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Hydrazine (35% by weight in water, 0.67 mL, 7.2 mmol) and 10% Pd/C (38 mg, 0.03 mmol) are added to a solution of 1-isopropyl-4-(4-nitrophenyl)piperidine (180 mg, 0.72 mmol) in EtOH (10 mL) and the mixture is heated at reflux for 3 h. After cooling, the mixture is filtered through celite and the solvent evaporated. The ...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
C1CC[NH]CC1.c1ccccc1
Other
[Pd].CCO
null
null
CC(C)N1CCC(c2ccc([N+](=O)[O-])cc2)CC1>[Pd].CCO>CC(C)N1CCC(c2ccc(N)cc2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e23b0e2df6e24238abf41bf5301133be
Brc1ncc(Br)n2ncnc12.CC(C)N1CCC(c2ccc(N)cc2)CC1>>CC(C)N1CCC(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)CC1
C(C)(C)N(C(C)C)CC.C(C)(C)N1CCC(CC1)C1=CC=C(C=C1)N.BrC1=CN=C(C=2N1N=CN2)Br>>BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)C2CCN(CC2)C(C)C
Br[c:13]1[n:14][cH:15][c:16]([Br:17])[n:18]2[n:19][cH:20][n:21][c:22]12.[CH3:1][CH:2]([CH3:3])[N:4]1[CH2:5][CH2:6][CH:7]([c:8]2[cH:9][cH:10][c:11]([NH2:12])[cH:23][cH:24]2)[CH2:25][CH2:26]1>>[CH3:1][CH:2]([CH3:3])[N:4]1[CH2:5][CH2:6][CH:7]([c:8]2[cH:9][cH:10][c:11]([NH:12][c:13]3[n:14][cH:15][c:16]([Br:17])[n:18]4[n:19...
Brc1ncc(Br)n2ncnc12.CC(C)N1CCC(c2ccc(N)cc2)CC1
CC(C)N1CCC(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)CC1
null
null
CC(C)O
Heteroatom Alkylation and Arylation
N-arylation (Buchwald-Hartwig/Ullmann-Goldberg)
aecfb0ede2c5d7901fea69101287828edf21f7a6e48b6ff83fe43de0688f1ef1
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1cn2ncnc2c(Nc2ccc(C3CCNCC3)cc2)n1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:1.[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[c:12]:[c:11](-[NH;D2;+0:10]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:1):[c:13]
null
[]
null
null
null
null
N,N-Diisopropylethylamine (200 μL, 1.2 mmol) is added to a mixture of 4-(1-isopropylpiperidin-4-yl)phenylamine (220 mg, 1.0 mmol) and 5,8-dibromo-[1,2,4]triazolo[1,5-a]pyrazine (280 mg, 1.0 mmol) in iPrOH (5 mL) and heated at reflux for 48 h. The mixture is cooled and the solvent evaporated under reduced pressure to af...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1cn2ncnc2cn1
c1cn2ncnc2cn1
C1CC[NH]CC1.c1ccccc1.c1cn2ncnc2cn1
HBr
CC(C)O
null
null
Brc1ncc(Br)n2ncnc12.CC(C)N1CCC(c2ccc(N)cc2)CC1>CC(C)O>CC(C)N1CCC(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d3d356812b1f43bf9733b56ece81d4c4
CC(C)(C)OC(=O)N1CCNC(=O)C1.Nc1ccc(I)cc1>>CC(C)(C)OC(=O)N1CCN(c2ccc(N)cc2)C(=O)C1
IC1=CC=C(N)C=C1.C(C)(C)(C)OC(=O)N1CC(NCC1)=O.C(=O)([O-])[O-].[K+].[K+]>>C(C)(C)(C)OC(=O)N1CC(N(CC1)C1=CC=C(C=C1)N)=O
[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[N:8]1[CH2:9][CH2:10][NH:11][C:19](=[O:20])[CH2:21]1.I[c:12]1[cH:13][cH:14][c:15]([NH2:16])[cH:17][cH:18]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[N:8]1[CH2:9][CH2:10][N:11]([c:12]2[cH:13][cH:14][c:15]([NH2:16])[cH:17][cH:18]2)[C:19](=[O:20])[CH2:21]1
CC(C)(C)OC(=O)N1CCNC(=O)C1.Nc1ccc(I)cc1
CC(C)(C)OC(=O)N1CCN(c2ccc(N)cc2)C(=O)C1
null
[Cu]I
O1CCOCC1
Heteroatom Alkylation and Arylation
Goldberg coupling
5cf9fe2d19ef8ad0958a3c8d70022b236c24bed4db0b46e16406f2c36d7c335f
e3642f27d4c4bc101b8817e43c6aa5a22f60531030ee51c1c76056fd17c8df37
O=C1CNCCN1c1ccccc1
I-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[O;D1;H0:6]=[C:7]1-[C:8]-[#7:9]-[C:10]-[C:11]-[NH;D2;+0:12]-1>>[O;D1;H0:6]=[C:7]1-[C:8]-[#7:9]-[C:10]-[C:11]-[N;H0;D3;+0:12]-1-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
87
[{"value": 87.0, "product": "C(C)(C)(C)OC(=O)N1CC(N(CC1)C1=CC=C(C=C1)N)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 86.6, "product": "C(C)(C)(C)OC(=O)N1CC(N(CC1)C1=CC=C(C=C1)N)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
119
CELSIUS
null
null
A suspension of p-iodo-aniline (918 mg, 4.8 mmol), 3-oxo-piperazine-1-carboxylic acid tert-butyl ester (960 mg, 4.2 mmol) (1R,2R)-cyclohexane-1,2-diamine (0.05 mL, 0.42 mmol), copper (I) iodide (14.9 mg, 0.0042 mmol) and K2CO3 (1.19 g, 2.04 mmol) in dioxane (4 mL), is purged with nitrogen for 5 min in a reaction tube. ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Secondary amide
Tertiary amide
C1C[NH]CCN1.c1ccccc1
C1C[NH]CC[NH]1.c1ccccc1
C1C[NH]CC[NH]1.c1ccccc1
HI
[Cu]I.O1CCOCC1
119
null
CC(C)(C)OC(=O)N1CCNC(=O)C1.Nc1ccc(I)cc1>[Cu]I.O1CCOCC1>CC(C)(C)OC(=O)N1CCN(c2ccc(N)cc2)C(=O)C1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-656a55838efe46668d7934a03825cb9b
Brc1ncc(Br)n2ncnc12.CC(C)(C)OC(=O)N1CCN(c2ccc(N)cc2)C(=O)C1>>CC(C)(C)OC(=O)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)C(=O)C1
C(C)N(C(C)C)C(C)C.CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2.BrC1=CN=C(C=2N1N=CN2)Br.C(C)(C)(C)OC(=O)N1CC(N(CC1)C1=CC=C(C=C1)N)=O>>C(C)(C)(C)OC(=O)N1CC(N(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)Br)N=CN2)=O
Br[c:17]1[n:18][cH:19][c:20]([Br:21])[n:22]2[n:23][cH:24][n:25][c:26]12.[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[N:8]1[CH2:9][CH2:10][N:11]([c:12]2[cH:13][cH:14][c:15]([NH2:16])[cH:27][cH:28]2)[C:29](=[O:30])[CH2:31]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[N:8]1[CH2:9][CH2:10][N:11]([c:12]2[cH:13][cH...
Brc1ncc(Br)n2ncnc12.CC(C)(C)OC(=O)N1CCN(c2ccc(N)cc2)C(=O)C1
CC(C)(C)OC(=O)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)C(=O)C1
null
null
CC(C)O
Heteroatom Alkylation and Arylation
N-arylation (Buchwald-Hartwig/Ullmann-Goldberg)
aecfb0ede2c5d7901fea69101287828edf21f7a6e48b6ff83fe43de0688f1ef1
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
O=C1CNCCN1c1ccc(Nc2nccn3ncnc23)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:1.[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[c:12]:[c:11](-[NH;D2;+0:10]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:1):[c:13]
51.6
[{"value": 51.0, "product": "C(C)(C)(C)OC(=O)N1CC(N(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)Br)N=CN2)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 51.6, "product": "C(C)(C)(C)OC(=O)N1CC(N(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)Br)N=CN2)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound may be prepared using methods as described for Compound 6, step 1, using 5,8-dibromo-[1,2,4]triazolo[1,5-a]pyrazine (0.283 g, 1.00 mmol), 4-(4-amino-phenyl)-3-oxo-piperazine-1-carboxylic acid ter-t-butyl ester (0.300 g, 1.00 mmol) and N-ethyldiisopropyl-amine (0.20 mL, 1.02 mmol) in 2-propanol (1 mL). Pur...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1cn2ncnc2cn1
c1cn2ncnc2cn1
C1C[NH]CC[NH]1.c1ccccc1.c1cn2ncnc2cn1
HBr
CC(C)O
null
null
Brc1ncc(Br)n2ncnc12.CC(C)(C)OC(=O)N1CCN(c2ccc(N)cc2)C(=O)C1>CC(C)O>CC(C)(C)OC(=O)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)C(=O)C1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-80745bb0fef4445eb6ea2a08f0aacb4d
CC(C)(C)OC(=O)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)C(=O)C1>>O=C1CNCCN1c1ccc(Nc2ncc(Br)n3ncnc23)cc1
C(C)(C)(C)OC(=O)N1CC(N(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)Br)N=CN2)=O.C(=O)(C(F)(F)F)O>>BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2C(CNCC2)=O
CC(C)(C)OC(=O)[N:4]1[CH2:3][C:2](=[O:1])[N:7]([c:8]2[cH:9][cH:10][c:11]([NH:12][c:13]3[n:14][cH:15][c:16]([Br:17])[n:18]4[n:19][cH:20][n:21][c:22]34)[cH:23][cH:24]2)[CH2:6][CH2:5]1>>[O:1]=[C:2]1[CH2:3][NH:4][CH2:5][CH2:6][N:7]1[c:8]1[cH:9][cH:10][c:11]([NH:12][c:13]2[n:14][cH:15][c:16]([Br:17])[n:18]3[n:19][cH:20][n:21...
CC(C)(C)OC(=O)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)C(=O)C1
O=C1CNCCN1c1ccc(Nc2ncc(Br)n3ncnc23)cc1
null
null
C(Cl)Cl.C(=O)(O)[O-].[Na+]
Reduction
Boc amine deprotection
2c25e19aee181a3c5131cfdfda27035fd54d4379a11d745dfb75d386bacfd500
a94b29c7264c852156fc1cdd4a0951a4fc26c06d0edc9e50c743825dbf79e3fd
O=C1CNCCN1c1ccc(Nc2nccn3ncnc23)cc1
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1]1-[C:2]-[C:3](=[O;D1;H0:4])-[#7:5](-[c:6])-[C:7]-[C:8]-1>>[O;D1;H0:4]=[C:3]1-[C:2]-[NH;D2;+0:1]-[C:8]-[C:7]-[#7:5]-1-[c:6]
78
[{"value": 78.0, "product": "BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2C(CNCC2)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 77.3, "product": "BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2C(CNCC2)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 4-[4-(5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-ylamino)-phenyl]-3-oxo-piperazine-1-carboxylic acid tert-butyl ester (0.252 mg, 0.6 mmol) in 2:1 DCM:TFA (4.8 mL) is stirred for 1 hour at room temperature. The mixture is then diluted with DCM and basified with sat. NaHCO3. The aqueous layer is extracted with...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Secondary amine
C1C[NH]CC[NH]1
C1C[NH]CCN1
C1C[NH]CCN1.c1ccccc1.c1cn2ncnc2cn1
HO-
C(Cl)Cl.C(=O)(O)[O-].[Na+]
null
null
CC(C)(C)OC(=O)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)C(=O)C1>C(Cl)Cl.C(=O)(O)[O-].[Na+]>O=C1CNCCN1c1ccc(Nc2ncc(Br)n3ncnc23)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-21d7e71ccb9b49acb3c3525c5cab7017
O=C1CNCCN1c1ccc(Nc2ncc(Br)n3ncnc23)cc1.c1nc2c(Nc3ccc(N4CCOCC4)cc3)ncc(-c3cn[nH]c3)n2n1>>O=C1CNCCN1c1ccc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)cc1
CC(C)(C)[O-].[Na+].N1(CCOCC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=NNC1)N=CN2.BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2C(CNCC2)=O>>N1N=CC(=C1)C1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2C(CNCC2)=O
Brc1cnc(Nc2c[cH:9][c:8]([N:7]3[C:2](=[O:1])[CH2:3][NH:4][CH2:5][CH2:6]3)[cH:28]c2)c2ncnn12.c1c(N2CCOCC2)c[cH:27][c:11]([NH:12][c:13]2[n:14][cH:15][c:16](-[c:17]3[cH:18][n:19][nH:20][cH:21]3)[n:22]3[n:23][cH:24][n:25][c:26]23)[cH:10]1>>[O:1]=[C:2]1[CH2:3][NH:4][CH2:5][CH2:6][N:7]1[c:8]1[cH:9][cH:10][c:11]([NH:12][c:13]2...
O=C1CNCCN1c1ccc(Nc2ncc(Br)n3ncnc23)cc1.c1nc2c(Nc3ccc(N4CCOCC4)cc3)ncc(-c3cn[nH]c3)n2n1
O=C1CNCCN1c1ccc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)cc1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
CN(C)C=O.O
Miscellaneous
OtherReaction
86ecf812006a71792fe0a5822d3580759e0bfe8f15868886516d1b5aead83a91
5e679d678442c10fe854b5580e44307cb1ba209a72c7b73f1ab7c0561ae39bd8
O=C1CNCCN1c1ccc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)cc1
Br-c1:c:n:c(-N-c2:c:[cH;D2;+0:1]:[c:2](-[#7:3]-[C:4]=[O;D1;H0:5]):[cH;D2;+0:6]:c:2):c2:n:c:n:n:1:2.[#7:7]-[c:8]1:[cH;D2;+0:9]:c:c(-N2-C-C-O-C-C-2):c:[cH;D2;+0:10]:1>>[#7:7]-[c:8]1:[cH;D2;+0:9]:[cH;D2;+0:6]:[c:2](-[#7:3]-[C:4]=[O;D1;H0:5]):[cH;D2;+0:1]:[cH;D2;+0:10]:1
19
[{"value": 19.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound may be prepared using methods as described for Compound 1, step 5 using 1-[4-(5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-ylamino)-phenyl]-piperazin-2-one (70 mg, 0.18 mmol) 4-(4,4,5,5-tetramethyl-1,3,2-dioxaborolan-2-yl)-1H-pyrazole (64 mg, 0.33 mmol), Pd(PPh3)4 (21 mg, 18 μmol) and NaOtBu (70 mg, 0.72 mmol)...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ether.Secondary amine.Tertiary amine
null
c1ccccc1.c1cn2ncnc2cn1.c1ccccc1.C1COCCN1
c1ccccc1
C1C[NH]CCN1.c1ccccc1.c1cn[nH]c1.c1cn2ncnc2cn1
HBr
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.CN(C)C=O.O
null
null
O=C1CNCCN1c1ccc(Nc2ncc(Br)n3ncnc23)cc1.c1nc2c(Nc3ccc(N4CCOCC4)cc3)ncc(-c3cn[nH]c3)n2n1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.CN(C)C=O.O>O=C1CNCCN1c1ccc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3854d07172e940f88e508a0d34f2519e
CC(C)(C)N1CCNCC1.O=[N+]([O-])c1ccc(F)cc1>>CC(C)(C)N1CCN(c2ccc([N+](=O)[O-])cc2)CC1.N
FC1=CC=C(C=C1)[N+](=O)[O-].C(C)(C)(C)N1CCNCC1.C(=O)([O-])[O-].[K+].[K+]>>N.C(C)(C)(C)N1CCN(CC1)C1=CC=C(C=C1)[N+](=O)[O-]
[CH3:1][C:2]([CH3:3])([CH3:4])[N:5]1[CH2:6][CH2:7][NH:8][CH2:18][CH2:19]1.F[c:9]1[cH:10][cH:11][c:12]([N+:13](=[O:14])[O-:15])[cH:16][cH:17]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[N:5]1[CH2:6][CH2:7][N:8]([c:9]2[cH:10][cH:11][c:12]([N+:13](=[O:14])[O-:15])[cH:16][cH:17]2)[CH2:18][CH2:19]1.[NH3:20]
CC(C)(C)N1CCNCC1.O=[N+]([O-])c1ccc(F)cc1
CC(C)(C)N1CCN(c2ccc([N+](=O)[O-])cc2)CC1.N
null
null
O1CCOCC1
Functional Group Interconversion
Buchwald-Hartwig/Ullmann-Goldberg/N-arylation secondary amine
c6c38d29142a1aca5d86f02d4b0c2562460ca1aec33aa213f11cd4062c6e7363
39ece5c8e1ec3e350cfadd8e37bb010493b934313e1cd5367f16de670d62b5af
c1ccc(N2CCNCC2)cc1
F-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[#7:6]1-[C:7]-[C:8]-[NH;D2;+0:9]-[C:10]-[C:11]-1>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[N;H0;D3;+0:9]1-[C:8]-[C:7]-[#7:6]-[C:11]-[C:10]-1):[c:4]:[c:5]
118.5
[{"value": 55.4, "product": "C(C)(C)(C)N1CCN(CC1)C1=CC=C(C=C1)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 118.5, "product": "C(C)(C)(C)N1CCN(CC1)C1=CC=C(C=C1)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
130
CELSIUS
8
HOUR
To a solution of 1-fluoro-4-nitro-benzene (314 mg, 2.23 mmol) and 4-tert-butyl-piperazine (1 g, 3.34 mmol) in dioxane (15 mL) is added K2CO3 (1.65 mg, 11.9 mmol) and the reaction is stirred at 130° C. overnight. The solvent is evaporated under vacuum and the residue is partitioned between ethyl acetate and water. The o...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Secondary amine
Tertiary amine
C1C[NH]CCN1.c1ccccc1
C1C[NH]CC[NH]1.c1ccccc1
C1C[NH]CC[NH]1.c1ccccc1
null
O1CCOCC1
130
8
CC(C)(C)N1CCNCC1.O=[N+]([O-])c1ccc(F)cc1>O1CCOCC1>CC(C)(C)N1CCN(c2ccc([N+](=O)[O-])cc2)CC1.N
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-fbaea089ba5241909d095e7297b4658b
CC(C)(C)N1CCN(c2ccc([N+](=O)[O-])cc2)CC1>>CC(C)(C)N1CCN(c2ccc(N)cc2)CC1
C(C)(C)(C)N1CCN(CC1)C1=CC=C(C=C1)[N+](=O)[O-].O.O.[Sn](Cl)Cl.Cl>>C(C)(C)(C)N1CCN(CC1)C1=CC=C(C=C1)N
O=[N+:13]([O-])[c:12]1[cH:11][cH:10][c:9]([N:8]2[CH2:7][CH2:6][N:5]([C:2]([CH3:1])([CH3:3])[CH3:4])[CH2:17][CH2:16]2)[cH:15][cH:14]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[N:5]1[CH2:6][CH2:7][N:8]([c:9]2[cH:10][cH:11][c:12]([NH2:13])[cH:14][cH:15]2)[CH2:16][CH2:17]1
CC(C)(C)N1CCN(c2ccc([N+](=O)[O-])cc2)CC1
CC(C)(C)N1CCN(c2ccc(N)cc2)CC1
null
null
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc(N2CCNCC2)cc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
100
[{"value": 99.0, "product": "C(C)(C)(C)N1CCN(CC1)C1=CC=C(C=C1)N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 100.0, "product": "C(C)(C)(C)N1CCN(CC1)C1=CC=C(C=C1)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
40
CELSIUS
8
HOUR
1-tert-Butyl-4-(4-nitro-phenyl)-piperazine (348 mg, 1.32 mmol) is dissolved in MeOH (10 mL) and tin (II) dichloride dihydrate (1.08 g, 4.79 mmol) is added. The mixture is cooled using a water bath and conc. HCl is added (3 mL). The reaction is stirred at 40° C. overnight. After removing the methanol, the resultant solu...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
C1C[NH]CC[NH]1.c1ccccc1
Other
CO
40
8
CC(C)(C)N1CCN(c2ccc([N+](=O)[O-])cc2)CC1>CO>CC(C)(C)N1CCN(c2ccc(N)cc2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6e039fcd201442198ed4aec7b55f7875
Brc1ncc(Br)n2ncnc12.CC(C)(C)N1CCN(c2ccc(N)cc2)CC1>>CC(C)(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)CC1
C(C)N(C(C)C)C(C)C.CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2.BrC1=CN=C(C=2N1N=CN2)Br.C(C)(C)(C)N1CCN(CC1)C1=CC=C(C=C1)N>>BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2CCN(CC2)C(C)(C)C
Br[c:14]1[n:15][cH:16][c:17]([Br:18])[n:19]2[n:20][cH:21][n:22][c:23]12.[CH3:1][C:2]([CH3:3])([CH3:4])[N:5]1[CH2:6][CH2:7][N:8]([c:9]2[cH:10][cH:11][c:12]([NH2:13])[cH:24][cH:25]2)[CH2:26][CH2:27]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[N:5]1[CH2:6][CH2:7][N:8]([c:9]2[cH:10][cH:11][c:12]([NH:13][c:14]3[n:15][cH:16][c:17]([Br:...
Brc1ncc(Br)n2ncnc12.CC(C)(C)N1CCN(c2ccc(N)cc2)CC1
CC(C)(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)CC1
null
null
CC(C)O
Heteroatom Alkylation and Arylation
N-arylation (Buchwald-Hartwig/Ullmann-Goldberg)
aecfb0ede2c5d7901fea69101287828edf21f7a6e48b6ff83fe43de0688f1ef1
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1cn2ncnc2c(Nc2ccc(N3CCNCC3)cc2)n1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:1.[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[c:12]:[c:11](-[NH;D2;+0:10]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:1):[c:13]
92.4
[{"value": 92.0, "product": "BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2CCN(CC2)C(C)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 92.4, "product": "BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2CCN(CC2)C(C)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound may be prepared using methods as described for Compound 6, step 1, using 5,8-dibromo-[1,2,4]triazolo[1,5-a]pyrazine (0.308 g, 1.107 mmol), 4-(4-tert-butyl-piperazin-1-yl)-phenylamine (0.310 g, 1.33 mmol) and N-ethyldiisopropyl-amine (0.289 mL, 1.66 mmol) in 2-propanol (5 mL). The reaction mixture is parti...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1cn2ncnc2cn1
c1cn2ncnc2cn1
C1C[NH]CC[NH]1.c1ccccc1.c1cn2ncnc2cn1
HBr
CC(C)O
null
null
Brc1ncc(Br)n2ncnc12.CC(C)(C)N1CCN(c2ccc(N)cc2)CC1>CC(C)O>CC(C)(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-792bf973e1ed4f4098679685b4aba99b
CC(C)(C)OC(=O)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)C(=O)C1.CC1(C)OB(c2ccc3c(c2)CNC3=O)OC1(C)C>>CC(C)(C)OC(=O)N1CCN(c2ccc(Nc3ncc(-c4ccc5c(c4)CNC5=O)n4ncnc34)cc2)C(=O)C1
CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2.CC1(OB(OC1(C)C)C=1C=C2CNC(C2=CC1)=O)C.C(=O)([O-])[O-].[Na+].[Na+].C(C)(C)(C)OC(=O)N1CC(N(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)Br)N=CN2)=O>>C(C)(C)(C)OC(=O)N1CC(N(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C3CNC(C3=CC1)=O)N=CN2)=O
Br[c:20]1[cH:19][n:18][c:17]([NH:16][c:15]2[cH:14][cH:13][c:12]([N:11]3[CH2:10][CH2:9][N:8]([C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[CH2:40][C:38]3=[O:39])[cH:37][cH:36]2)[c:35]2[n:31]1[n:32][cH:33][n:34]2.CC1(C)OB([c:21]2[cH:22][cH:23][c:24]3[c:25]([cH:26]2)[CH2:27][NH:28][C:29]3=[O:30])OC1(C)C>>[CH3:1][C:2](...
CC(C)(C)OC(=O)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)C(=O)C1.CC1(C)OB(c2ccc3c(c2)CNC3=O)OC1(C)C
CC(C)(C)OC(=O)N1CCN(c2ccc(Nc3ncc(-c4ccc5c(c4)CNC5=O)n4ncnc34)cc2)C(=O)C1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O1CCOCC1.C1(=CC=CC=C1)C.[Cl-].[Na+].O
C-C Coupling
Suzuki coupling with boronic esters
0e514a9992c96da29f2ec2414679fb7906a3f635b15b1ade3e33600ae6778418
b42efb3b6a7742d5af594c6a3031e487327e58e9f8c2f428ee68996c98377910
O=C1NCc2cc(-c3cnc(Nc4ccc(N5CCNCC5=O)cc4)c4ncnn34)ccc21
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1.C-C1(-C)-O-B(-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14])-O-C-1(-C)-C>>[c:12]:[c:11]:[c;H0;D3;+0:10](-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1):[c:13]:[c:14]
47
[{"value": 47.0, "product": "C(C)(C)(C)OC(=O)N1CC(N(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C3CNC(C3=CC1)=O)N=CN2)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 46.2, "product": "C(C)(C)(C)OC(=O)N1CC(N(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C3CNC(C3=CC1)=O)N=CN2)=O", "details": "CALCULATEDPERCENTYIELD", "...
null
null
null
null
This compound may be prepared using methods as described for Compound 6, step 4, using 4-[4-(5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-ylamino)-phenyl]-3-oxo-piperazine-1-carboxylic acid tert-butyl ester (115 mg, 0.24 mmol), 5-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-2,3-dihydro-isoindol-1-one (92 mg, 0.35 mmol), a...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic ester
null
c1cn2ncnc2cn1.B1OCCO1.c1ccc2c(c1)CNC2
c1ccc2c(c1)CNC2.c1cn2ncnc2cn1
C1C[NH]CC[NH]1.c1ccccc1.c1ccc2c(c1)CNC2.c1cn2ncnc2cn1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1.C1(=CC=CC=C1)C.[Cl-].[Na+].O
null
null
CC(C)(C)OC(=O)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)C(=O)C1.CC1(C)OB(c2ccc3c(c2)CNC3=O)OC1(C)C>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1.C1(=CC=CC=C1)C.[Cl-].[Na+].O>CC(C)(C)OC(=O)N1CCN...
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3a63ddd80d1743edae2443277d01f2d4
CC(C)(C)OC(=O)N1CCN(c2ccc(Nc3ncc(-c4ccc5c(c4)CNC5=O)n4ncnc34)cc2)C(=O)C1>>O=C1NCc2cc(-c3cnc(Nc4ccc(N5CCNCC5=O)cc4)c4ncnn34)ccc21
C(C)(C)(C)OC(=O)N1CC(N(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C3CNC(C3=CC1)=O)N=CN2)=O.C(=O)(C(F)(F)F)O>>O=C1N(CCNC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C3CNC(C3=CC1)=O)N=CN2
CC(C)(C)OC(=O)[N:20]1[CH2:19][CH2:18][N:17]([c:16]2[cH:15][cH:14][c:13]([NH:12][c:11]3[n:10][cH:9][c:8](-[c:7]4[cH:6][c:5]5[c:33]([cH:32][cH:31]4)[C:2](=[O:1])[NH:3][CH2:4]5)[n:30]4[c:26]3[n:27][cH:28][n:29]4)[cH:25][cH:24]2)[C:22](=[O:23])[CH2:21]1>>[O:1]=[C:2]1[NH:3][CH2:4][c:5]2[cH:6][c:7](-[c:8]3[cH:9][n:10][c:11](...
CC(C)(C)OC(=O)N1CCN(c2ccc(Nc3ncc(-c4ccc5c(c4)CNC5=O)n4ncnc34)cc2)C(=O)C1
O=C1NCc2cc(-c3cnc(Nc4ccc(N5CCNCC5=O)cc4)c4ncnn34)ccc21
null
null
C(Cl)Cl.C(=O)(O)[O-].[Na+]
Reduction
Boc amine deprotection
2c25e19aee181a3c5131cfdfda27035fd54d4379a11d745dfb75d386bacfd500
a94b29c7264c852156fc1cdd4a0951a4fc26c06d0edc9e50c743825dbf79e3fd
O=C1NCc2cc(-c3cnc(Nc4ccc(N5CCNCC5=O)cc4)c4ncnn34)ccc21
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1]1-[C:2]-[C:3]-[#7:4](-[c:5])-[C:6](=[O;D1;H0:7])-[C:8]-1>>[O;D1;H0:7]=[C:6]1-[C:8]-[NH;D2;+0:1]-[C:2]-[C:3]-[#7:4]-1-[c:5]
86.3
[{"value": 86.0, "product": "O=C1N(CCNC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C3CNC(C3=CC1)=O)N=CN2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 86.3, "product": "O=C1N(CCNC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C3CNC(C3=CC1)=O)N=CN2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 3-oxo-4-{4-[5-(1-oxo-2,3-dihydro-1H-isoindol-5-yl)-[1,2,4]triazolo[1,5-a]pyrazin-8-ylamino]-phenyl}-piperazine-1-carboxylic acid tert-butyl ester (59 mg, 0.1 mmol) in 3:1 DCM:TFA (1.2 mL) is stirred at room temperature for 1 hour. The reaction mixture is diluted with DCM and basified with sat. NaHCO3. The...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Secondary amine
C1C[NH]CC[NH]1
C1C[NH]CCN1
c1ccc2c(c1)CNC2.c1ccccc1.C1C[NH]CCN1.c1cn2ncnc2cn1
HO-
C(Cl)Cl.C(=O)(O)[O-].[Na+]
null
null
CC(C)(C)OC(=O)N1CCN(c2ccc(Nc3ncc(-c4ccc5c(c4)CNC5=O)n4ncnc34)cc2)C(=O)C1>C(Cl)Cl.C(=O)(O)[O-].[Na+]>O=C1NCc2cc(-c3cnc(Nc4ccc(N5CCNCC5=O)cc4)c4ncnn34)ccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3d0cc6449da24f45998160c2fbd1552d
CN(C)C=O.O=C(O)c1c(F)cc(Br)cc1F>>COC(=O)c1c(F)cc(Br)cc1F
Cl.S(=O)(Cl)Cl.CN(C)C=O.BrC1=CC(=C(C(=O)O)C(=C1)F)F>>COC(C1=C(C=C(C=C1F)Br)F)=O
CN(C=O)[CH3:1].[OH:2][C:3](=[O:4])[c:5]1[c:6]([F:7])[cH:8][c:9]([Br:10])[cH:11][c:12]1[F:13]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[c:6]([F:7])[cH:8][c:9]([Br:10])[cH:11][c:12]1[F:13]
CN(C)C=O.O=C(O)c1c(F)cc(Br)cc1F
COC(=O)c1c(F)cc(Br)cc1F
null
null
C(Cl)Cl.CO
Heteroatom Alkylation and Arylation
O-methylation
c9172060953e4f6c47363a85681e8adf6b8a08eda11980515725076232558272
897317edf82e08b628c69c2b6ae6e330cef34fadcc7a095baba8a1e1a8ad34d6
c1ccccc1
C-N(-[CH3;D1;+0:1])-C=O.[O;D1;H0:2]=[C:3](-[OH;D1;+0:4])-[c:5]>>[CH3;D1;+0:1]-[O;H0;D2;+0:4]-[C:3](=[O;D1;H0:2])-[c:5]
null
[]
null
null
2.5
HOUR
To a suspension of 4-Bromo-2,6-difluoro-benzoic acid (5 g, 21 mmol) in DCM (10 mL) is added thionyl chloride (15 mL) and DMF (0.5 mL). The mixture is stirred at room temperature for 2.5 h. It is then cooled to 0° C. and MeOH (20 mL) is added carefully causing vigorous HCl evolution. After stirring for an additional 0.5...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Tertiary amide
Ester
null
null
c1ccccc1
HO-
C(Cl)Cl.CO
null
2.5
CN(C)C=O.O=C(O)c1c(F)cc(Br)cc1F>C(Cl)Cl.CO>COC(=O)c1c(F)cc(Br)cc1F
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2cbdcdb2a20b4923b72160aca7919a86
COC(=O)c1c(F)cc(Br)cc1F.C[N+](=O)[O-]>>COC(=O)c1c(F)cc(Br)cc1C[N+](=O)[O-]
COC(C1=C(C=C(C=C1F)Br)F)=O.[N+](=O)([O-])C.[H-].[Na+].[O-]S(=O)(=O)[O-].[Mg+2]>>COC(C1=C(C=C(C=C1C[N+](=O)[O-])Br)F)=O
F[c:12]1[c:5]([C:3]([O:2][CH3:1])=[O:4])[c:6]([F:7])[cH:8][c:9]([Br:10])[cH:11]1.[CH3:13][N+:14](=[O:15])[O-:16]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[c:6]([F:7])[cH:8][c:9]([Br:10])[cH:11][c:12]1[CH2:13][N+:14](=[O:15])[O-:16]
COC(=O)c1c(F)cc(Br)cc1F.C[N+](=O)[O-]
COC(=O)c1c(F)cc(Br)cc1C[N+](=O)[O-]
null
null
CS(=O)C
C-C Coupling
OtherReaction
cd8b5052688b7919a207207149d12f6b6cbbc3b607c9eb9fde3a8ff930782506
5dcf4124513b16cd3f4b18ce2434242a66d25ddc466fbc0674492d31d46556fb
c1ccccc1
F-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[C:5](=[O;D1;H0:6])-[#8:7]-[C;D1;H3:8]):[c:9].[CH3;D1;+0:10]-[#7;+:11](-[O;-;D1;H0:12])=[O;D1;H0:13]>>[C;D1;H3:8]-[#8:7]-[C:5](=[O;D1;H0:6])-[c:4](:[c:9]):[c;H0;D3;+0:1](-[CH2;D2;+0:10]-[#7;+:11](-[O;-;D1;H0:12])=[O;D1;H0:13]):[c:2]:[c:3]
null
[]
null
null
0.25
HOUR
Nitromethane (10 mL, 169 mmol, 8 equiv.) is added cautiously to a suspension of sodium hydride (4.05 g, 169 mmol, 8 equiv.) and MgSO4 (40 g) in DMSO (100 mL) at rt and the resulting slurry is stirred for 0.25 h. To the resulting yellow slurry is added 4-bromo-2,6-difluorobenzoic acid methyl ester (5.3 g, 21 mmol) and t...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Nitro group
Nitro group
c1ccccc1
c1ccccc1
c1ccccc1
HF
CS(=O)C
null
0.25
COC(=O)c1c(F)cc(Br)cc1F.C[N+](=O)[O-]>CS(=O)C>COC(=O)c1c(F)cc(Br)cc1C[N+](=O)[O-]
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d7a5d50cbcc84b2588b75eadef826e0e
COC(=O)c1c(F)cc(Br)cc1C[N+](=O)[O-]>>O=C1NCc2cc(Br)cc(F)c21
N.COC(C1=C(C=C(C=C1C[N+](=O)[O-])Br)F)=O.C(=O)[O-].[NH4+]>>BrC=1C=C2CNC(C2=C(C1)F)=O
CO[C:2](=[O:1])[c:12]1[c:5]([CH2:4][N+:3](=O)[O-])[cH:6][c:7]([Br:8])[cH:9][c:10]1[F:11]>>[O:1]=[C:2]1[NH:3][CH2:4][c:5]2[cH:6][c:7]([Br:8])[cH:9][c:10]([F:11])[c:12]21
COC(=O)c1c(F)cc(Br)cc1C[N+](=O)[O-]
O=C1NCc2cc(Br)cc(F)c21
null
[Zn]
C(Cl)Cl.CO
Functional Group Interconversion
OtherReaction
166d9d3d6afdc459f3b81568112cf297aeec7e6533dedd63b925cc3c46d90830
42f24d3b25bb26f4d7fac0ebbebf6d046ea37d400eb2e6f47c39069d069d5e9d
O=C1NCc2ccccc21
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]-[C:6]-[N+;H0;D3:7](=O)-[O-]>>[O;D1;H0:2]=[C;H0;D3;+0:1]1-[NH;D2;+0:7]-[C:6]-[c:5]:[c:3]-1:[c:4]
null
[]
null
null
0.3
HOUR
Crude 4-bromo-2-fluoro-6-(nitromethyl)benzoic acid methyl ester from the previous step is dissolved in MeOH (100 mL). To this clear orange solution is added Zinc dust (3.35 g, 51.3 mmol, 3 equiv.) followed by ammonium formate (3.23 g, 51.3 mmol, 3 equiv.) which results in an exothermic reaction. After 0.3 h, 7M NH3 in ...
10.6084/m9.figshare.5104873.v1
null
Ester.Nitro group
Secondary amide
null
c1ccc2c(c1)CNC2
c1ccc2c(c1)CNC2
HO-
[Zn].C(Cl)Cl.CO
null
0.3
COC(=O)c1c(F)cc(Br)cc1C[N+](=O)[O-]>[Zn].C(Cl)Cl.CO>O=C1NCc2cc(Br)cc(F)c21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-31b3761fa2b2411d9d9313462cee3b07
CC(C)=O.O=C1CNCCN1c1ccc(Nc2ncc(Br)n3ncnc23)cc1>>CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)C(=O)C1
Cl.[BH3-]C#N.[Na+].BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2C(CNCC2)=O.C(C)(=O)O.CC(=O)[O-].[Na+].CC(=O)C>>BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2C(CN(CC2)C(C)C)=O
O=[C:2]([CH3:1])[CH3:3].[NH:4]1[CH2:5][CH2:6][N:7]([c:8]2[cH:9][cH:10][c:11]([NH:12][c:13]3[n:14][cH:15][c:16]([Br:17])[n:18]4[n:19][cH:20][n:21][c:22]34)[cH:23][cH:24]2)[C:25](=[O:26])[CH2:27]1>>[CH3:1][CH:2]([CH3:3])[N:4]1[CH2:5][CH2:6][N:7]([c:8]2[cH:9][cH:10][c:11]([NH:12][c:13]3[n:14][cH:15][c:16]([Br:17])[n:18]4[...
CC(C)=O.O=C1CNCCN1c1ccc(Nc2ncc(Br)n3ncnc23)cc1
CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)C(=O)C1
null
null
CO
Heteroatom Alkylation and Arylation
reductive amination
d4cc9a2a46f538d7a2ff577eac4d4531ea828578c3aec2ccd0e8c1d501914fc6
99acf13bfcfe579f51ccb82c65e4ca039ee7ca9b6fcd2747a3d9a292a88e564e
O=C1CNCCN1c1ccc(Nc2nccn3ncnc23)cc1
O=[C;H0;D3;+0:1](-[C;D1;H3:2])-[C;D1;H3:3].[O;D1;H0:4]=[C:5]1-[C:6]-[NH;D2;+0:7]-[C:8]-[C:9]-[#7:10]-1-[c:11]>>[C;D1;H3:2]-[CH;D3;+0:1](-[C;D1;H3:3])-[N;H0;D3;+0:7]1-[C:6]-[C:5](=[O;D1;H0:4])-[#7:10](-[c:11])-[C:9]-[C:8]-1
25
[{"value": 25.0, "product": "BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2C(CN(CC2)C(C)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 22.3, "product": "BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2C(CN(CC2)C(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a solution of 1-[4-(5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-ylamino)-phenyl]-piperazin-2-one (example 31, step 2) (180 mg, 0.47 mmol) in MeOH (4 mL) are added acetic acid (0.03 mL, 0.47 mmol), NaOAc (38 mg, 0.47 mmol) and acetone (0.2 mL, 1.18 mmol). The reaction mixture is stirred at room temperature for 1 hour the...
10.6084/m9.figshare.5104873.v1
null
Ketone.Secondary amine
Tertiary amine
C1CNCC[NH]1
C1C[NH]CC[NH]1
C1C[NH]CC[NH]1.c1ccccc1.c1cn2ncnc2cn1
Other
CO
null
1
CC(C)=O.O=C1CNCCN1c1ccc(Nc2ncc(Br)n3ncnc23)cc1>CO>CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)C(=O)C1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4aa3a42f7ba04c6ca4b3d36ee16a900e
CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)C(=O)C1.CC1(C)OB(c2ccc3c(c2)CNC3=O)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1>>CC(C)N1CCN(c2ccc(Nc3ncc(-c4ccc5c(c4)CNC5=O)n4ncnc34)cc2)C(=O)C1.N
C(=O)([O-])[O-].[Na+].[Na+].BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2C(CN(CC2)C(C)C)=O.CC1(OB(OC1(C)C)C=1C=C2CNC(C2=CC1)=O)C.CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2>>N.C(C)(C)N1CC(N(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C3CNC(C3=CC1)=O)N=CN2)=O
Br[c:16]1[cH:15][n:14][c:13]([NH:12][c:11]2[cH:10][cH:9][c:8]([N:7]3[CH2:6][CH2:5][N:4]([CH:2]([CH3:1])[CH3:3])[CH2:36][C:34]3=[O:35])[cH:33][cH:32]2)[c:31]2[n:27]1[n:28][cH:29][n:30]2.CC1(C)OB([c:17]2[cH:18][cH:19][c:20]3[c:21]([cH:22]2)[CH2:23][NH:24][C:25]3=[O:26])OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(=O)[NH2:37])c4)...
CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)C(=O)C1.CC1(C)OB(c2ccc3c(c2)CNC3=O)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1
CC(C)N1CCN(c2ccc(Nc3ncc(-c4ccc5c(c4)CNC5=O)n4ncnc34)cc2)C(=O)C1.N
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O1CCOCC1.C1(=CC=CC=C1)C.[Cl-].[Na+].O
C-C Coupling
OtherReaction
d96e7a493e1619b343e6902e2f3e9ceea3531a747b8fbd8e81a720c753a845f2
96e5f3628c1bd4659dd3e9821904115decf673d0e8e42bb7900b7f521b084c51
O=C1NCc2cc(-c3cnc(Nc4ccc(N5CCNCC5=O)cc4)c4ncnn34)ccc21
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1.C-C1(-C)-O-B(-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14])-O-C-1(-C)-C.C-N1-C-C-N(-c2:c:c:c(-N-c3:n:c:c(-c4:c:s:c(-C(=O)-[NH2;D1;+0:15]):c:4):n4:n:c:n:c:3:4):c:c:2)-C-C-1>>[NH3;D0;+0:15].[c:12]:[c:11]:[c;H0;D3;+0:10](-[c;H0;D3;+0:1]1:...
55
[{"value": 55.0, "product": "C(C)(C)N1CC(N(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C3CNC(C3=CC1)=O)N=CN2)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound may be prepared using methods as described for Compound 6, step 4, using 1-[4-(5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-ylamino)-phenyl]-4-isopropyl-piperazin-2-one (40 mg, 0.09 mmol), 5-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-2,3-dihydro-isoindol-1-one (37 mg, 0.14 mmol), and Pd(PPh3)4 (31 mg, 0.02...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amide.Secondary amine.Tertiary amine.Tertiary amine.Boronic ester
null
c1cn2ncnc2cn1.B1OCCO1.c1ccc2c(c1)CNC2.C1CNCCN1.c1ccccc1.c1ccsc1.c1cn2ncnc2cn1
c1ccc2c(c1)CNC2.c1cn2ncnc2cn1
C1C[NH]CC[NH]1.c1ccccc1.c1ccc2c(c1)CNC2.c1cn2ncnc2cn1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1.C1(=CC=CC=C1)C.[Cl-].[Na+].O
null
null
CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)C(=O)C1.CC1(C)OB(c2ccc3c(c2)CNC3=O)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1.C1(...
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f2d8e5b64ea644f5b070681cb504cfdd
CI.COc1ccc(CBr)cc1.O=C1NCc2cc(Br)ccc21>>COc1ccc(CN2C(=O)c3ccc(Br)cc3C2(C)C)cc1
BrC=1C=C2CNC(C2=CC1)=O.C1CCOC1.[H-].[Na+].COC1=CC=C(CBr)C=C1.IC.[NH4+].[Cl-].[H-].[Na+].[I-].C1CCOC1>>BrC=1C=C2C(N(C(C2=CC1)=O)CC1=CC=C(C=C1)OC)(C)C
I[CH3:20].Br[CH2:7][c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:22][cH:21]1.[NH:8]1[C:9](=[O:10])[c:11]2[cH:12][cH:13][c:14]([Br:15])[cH:16][c:17]2[CH2:18]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][N:8]2[C:9](=[O:10])[c:11]3[cH:12][cH:13][c:14]([Br:15])[cH:16][c:17]3[C:18]2([CH3:19])[CH3:20])[cH:21][cH:22]1
CI.COc1ccc(CBr)cc1.O=C1NCc2cc(Br)ccc21
COc1ccc(CN2C(=O)c3ccc(Br)cc3C2(C)C)cc1
null
null
CN(C)C=O.C(C)(=O)OCC
Heteroatom Alkylation and Arylation
OtherReaction
9f5b0a1dbe0bd9f7211acdfdc653a03d59b835d4d029f835ea392c4ae188fa9a
4a6c1e88c9e8bed487b746792f88d478ff36cc235f9a217d4632e6babdebdc9a
O=C1c2ccccc2CN1Cc1ccccc1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].I-[CH3;D1;+0:5].[O;D1;H0:6]=[C:7]1-[NH;D2;+0:8]-[CH2;D2;+0:9]-[c:10](:[c:11]):[c:12]-1>>[C;D1;H3:13]-[C;H0;D4;+0:9]1(-[CH3;D1;+0:5])-[N;H0;D3;+0:8](-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4])-[C:7](=[O;D1;H0:6])-[c:12]:[c:10]-1:[c:11]
null
[]
null
null
4
HOUR
A suspension of sodium hydride (130 mg, 60% dispersion in mineral oil, 3.2 mmol) and tetra-nbutylammonium iodide (243 mg, 0.68 mmol) in THF (20 mL) is stirred at rt and a solution of 5-bromo-2,3-dihydroisoindol-1-one (675 mg, 3.2 mmol) in THF (20 mL) and DMF (4 mL) is added. After 75 min 4-methoxybenzyl bromide (460 μL...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amide
Tertiary amide
c1ccc2c(c1)CNC2
c1ccc2c(c1)C[NH]C2
c1ccccc1.c1ccc2c(c1)C[NH]C2
Br-.I-
CN(C)C=O.C(C)(=O)OCC
null
4
CI.COc1ccc(CBr)cc1.O=C1NCc2cc(Br)ccc21>CN(C)C=O.C(C)(=O)OCC>COc1ccc(CN2C(=O)c3ccc(Br)cc3C2(C)C)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3eae8be13edb415e92dc28b5f0766434
COc1ccc(CN2C(=O)c3ccc(Br)cc3C2(C)C)cc1>>CC1(C)NC(=O)c2ccc(Br)cc21
BrC=1C=C2C(N(C(C2=CC1)=O)CC1=CC=C(C=C1)OC)(C)C>>BrC=1C=C2C(NC(C2=CC1)=O)(C)C
COc1ccc(C[N:4]2[C:2]([CH3:1])([CH3:3])[c:13]3[c:7]([cH:8][cH:9][c:10]([Br:11])[cH:12]3)[C:5]2=[O:6])cc1>>[CH3:1][C:2]1([CH3:3])[NH:4][C:5](=[O:6])[c:7]2[cH:8][cH:9][c:10]([Br:11])[cH:12][c:13]21
COc1ccc(CN2C(=O)c3ccc(Br)cc3C2(C)C)cc1
CC1(C)NC(=O)c2ccc(Br)cc21
null
null
C(C)#N.O.C(C)(=O)OCC
Reduction
Hydrogenolysis of tertiary amines
e7566f8128c1a44807aeb07dea55552bf419d8005020ba5dabdef40b36726993
3da95258cd6a6ca6a5fed40d269eda3c543e9e67e5f33234974139a39c57d43d
O=C1NCc2ccccc21
C-O-c1:c:c:c(-C-[N;H0;D3;+0:1]2-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]-[C:6]-2(-[C;D1;H3:7])-[C;D1;H3:8]):c:c:1>>[C;D1;H3:7]-[C:6]1(-[C;D1;H3:8])-[NH;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]-1
86
[{"value": 86.0, "product": "BrC=1C=C2C(NC(C2=CC1)=O)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 5-bromo-2-(4-methoxybenzyl)-3,3-dimethyl-2,3-dihydroisoindol-1-one (640 mg, 1.78 mmol) and ceric ammonium nitrate (2.91 g, 5.33 mmol) in acetonitrile (11 mL) and water (5 mL) is stirred at 0° C. for 45 min. The solution is diluted with ethyl acetate (100 mL) and washed with brine (40 mL). The organic solv...
10.6084/m9.figshare.5104873.v1
null
Ether.Tertiary amide
Secondary amide
c1ccccc1.c1ccc2c(c1)C[NH]C2
c1ccc2c(c1)CNC2
c1ccc2c(c1)CNC2
HO-
C(C)#N.O.C(C)(=O)OCC
null
null
COc1ccc(CN2C(=O)c3ccc(Br)cc3C2(C)C)cc1>C(C)#N.O.C(C)(=O)OCC>CC1(C)NC(=O)c2ccc(Br)cc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-405bef0570904f9abc44789b427e7f09
CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)CC1.CC1(C)NC(=O)c2ccc(Br)cc21>>CC(C)N1CCN(c2ccc(Nc3ncc(-c4ccc5c(c4)C(C)(C)NC5=O)n4ncnc34)cc2)CC1
BrC=1C=C2C(NC(C2=CC1)=O)(C)C.B([O-])[O-].BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)N2CCN(CC2)C(C)C>>C(C)(C)N1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C3C(NC(C3=CC1)=O)(C)C)N=CN2
Br[c:16]1[cH:15][n:14][c:13]([NH:12][c:11]2[cH:10][cH:9][c:8]([N:7]3[CH2:6][CH2:5][N:4]([CH:2]([CH3:1])[CH3:3])[CH2:37][CH2:36]3)[cH:35][cH:34]2)[c:33]2[n:29]1[n:30][cH:31][n:32]2.Br[c:17]1[cH:18][cH:19][c:20]2[c:21]([cH:22]1)[C:23]([CH3:24])([CH3:25])[NH:26][C:27]2=[O:28]>>[CH3:1][CH:2]([CH3:3])[N:4]1[CH2:5][CH2:6][N:...
CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)CC1.CC1(C)NC(=O)c2ccc(Br)cc21
CC(C)N1CCN(c2ccc(Nc3ncc(-c4ccc5c(c4)C(C)(C)NC5=O)n4ncnc34)cc2)CC1
null
null
null
C-C Coupling
Negishi
beec43a7e9690bedf06a3f41502760638b5f58c8f2a5cf6eff7eca2c4f053fe6
a7a4ce9a92e2f8a62d28956a69a5cc384426ab72416e87d68c6a3feb23c22d66
O=C1NCc2cc(-c3cnc(Nc4ccc(N5CCNCC5)cc4)c4ncnn34)ccc21
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].Br-[c;H0;D3;+0:6]1:[c:7]:[#7;a:8]:[c:9]:[c:10]2:[#7;a:11]:[c:12]:[#7;a:13]:[#7;a:14]:2:1>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6]1:[c:7]:[#7;a:8]:[c:9]:[c:10]2:[#7;a:11]:[c:12]:[#7;a:13]:[#7;a:14]:2:1):[c:4]:[c:5]
null
[]
null
null
null
null
5-Bromo-3,3-dimethyl-2,3-dihydroisoindol-1-one is converted to the corresponding boronate in a fashion analogous to Intermediate 6, Step 3. This is then used to prepare the title compound from (5-bromo[1,2,4]triazolo[1,5-a]pyrazin-8-yl)-[4-(4-isopropylpiperazin-1-yl)-phenyl]amine using methods as described for Compound...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide
null
c1cn2ncnc2cn1.c1ccc2c(c1)CNC2
c1ccc2c(c1)CNC2.c1cn2ncnc2cn1
C1C[NH]CC[NH]1.c1ccccc1.c1ccc2c(c1)CNC2.c1cn2ncnc2cn1
Br-
null
null
null
CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2)CC1.CC1(C)NC(=O)c2ccc(Br)cc21>>CC(C)N1CCN(c2ccc(Nc3ncc(-c4ccc5c(c4)C(C)(C)NC5=O)n4ncnc34)cc2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9f5414befd6b43e4b8bf61b0c1b78428
Brc1ncc(Br)n2ncnc12.COC(=O)c1ccc(N)cc1>>COC(=O)c1ccc(Nc2ncc(Br)n3ncnc23)cc1
C(C)N(C(C)C)C(C)C.BrC1=CN=C(C=2N1N=CN2)Br.CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2.COC(C1=CC=C(C=C1)N)=O>>COC(C1=CC=C(C=C1)NC=1C=2N(C(=CN1)Br)N=CN2)=O
Br[c:10]1[n:11][cH:12][c:13]([Br:14])[n:15]2[n:16][cH:17][n:18][c:19]12.[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([NH2:9])[cH:20][cH:21]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([NH:9][c:10]2[n:11][cH:12][c:13]([Br:14])[n:15]3[n:16][cH:17][n:18][c:19]23)[cH:20][cH:21]1
Brc1ncc(Br)n2ncnc12.COC(=O)c1ccc(N)cc1
COC(=O)c1ccc(Nc2ncc(Br)n3ncnc23)cc1
null
null
CC(C)O
Heteroatom Alkylation and Arylation
N-arylation (Buchwald-Hartwig/Ullmann-Goldberg)
aecfb0ede2c5d7901fea69101287828edf21f7a6e48b6ff83fe43de0688f1ef1
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(Nc2nccn3ncnc23)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:1.[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[c:12]:[c:11](-[NH;D2;+0:10]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:1):[c:13]
null
[]
null
null
null
null
This compound may be prepared using methods as described for Compound 6, step 1 using 5,8-dibromo-[1,2,4]triazolo[1,5-a]pyrazine (250 mg, 0.90 mmol), 4-aminobenzoic methyl ester (163 mg, 1.08 mmol) and N-ethyldiisopropyl-amine (0.19 mL, 1.08 mmol) in 2-propanol (2.5 mL). The title compound is obtained after trituration...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1cn2ncnc2cn1
c1cn2ncnc2cn1
c1ccccc1.c1cn2ncnc2cn1
HBr
CC(C)O
null
null
Brc1ncc(Br)n2ncnc12.COC(=O)c1ccc(N)cc1>CC(C)O>COC(=O)c1ccc(Nc2ncc(Br)n3ncnc23)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2e1ed6dc46e549f8adcab4603cc91303
COC(=O)c1ccc(Nc2ncc(Br)n3ncnc23)cc1>>O=C(O)c1ccc(Nc2ncc(Br)n3ncnc23)cc1
COC(C1=CC=C(C=C1)NC=1C=2N(C(=CN1)Br)N=CN2)=O.O.[OH-].[Li+].CO>>BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C(=O)O)C=C2
C[O:3][C:2](=[O:1])[c:4]1[cH:5][cH:6][c:7]([NH:8][c:9]2[n:10][cH:11][c:12]([Br:13])[n:14]3[n:15][cH:16][n:17][c:18]23)[cH:19][cH:20]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][c:7]([NH:8][c:9]2[n:10][cH:11][c:12]([Br:13])[n:14]3[n:15][cH:16][n:17][c:18]23)[cH:19][cH:20]1
COC(=O)c1ccc(Nc2ncc(Br)n3ncnc23)cc1
O=C(O)c1ccc(Nc2ncc(Br)n3ncnc23)cc1
null
null
O.C1CCOC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(Nc2nccn3ncnc23)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]
49
[{"value": 49.0, "product": "BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C(=O)O)C=C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 48.7, "product": "BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C(=O)O)C=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
4-(5-Bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-ylamino)-benzoic acid methyl ester (460 mg, 1.32 mmol) is suspended in THF (11 mL) and a solution of lithium hydroxide monohydrate (554 mg, 13.2 mmol) in water (11 mL) is added. The reaction mixture is stirred at room temperature for 4 hours then methanol (11 mL) is added and ...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1cn2ncnc2cn1
Other
O.C1CCOC1
null
4
COC(=O)c1ccc(Nc2ncc(Br)n3ncnc23)cc1>O.C1CCOC1>O=C(O)c1ccc(Nc2ncc(Br)n3ncnc23)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b845953dd7eb40e0a2010114ce8d5640
NCc1cccnc1.O=C(O)c1ccc(Nc2ncc(Br)n3ncnc23)cc1>>O=C(NCc1cccnc1)c1ccc(Nc2ncc(Br)n3ncnc23)cc1
BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C(=O)O)C=C2.ON1N=NC2=C1C=CC=C2.O.C(C)N=C=NCCCN(C)C.N1=CC(=CC=C1)CN>>BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C(=O)NCC=1C=NC=CC1)C=C2
[NH2:3][CH2:4][c:5]1[cH:6][cH:7][cH:8][n:9][cH:10]1.O[C:2](=[O:1])[c:11]1[cH:12][cH:13][c:14]([NH:15][c:16]2[n:17][cH:18][c:19]([Br:20])[n:21]3[n:22][cH:23][n:24][c:25]23)[cH:26][cH:27]1>>[O:1]=[C:2]([NH:3][CH2:4][c:5]1[cH:6][cH:7][cH:8][n:9][cH:10]1)[c:11]1[cH:12][cH:13][c:14]([NH:15][c:16]2[n:17][cH:18][c:19]([Br:20]...
NCc1cccnc1.O=C(O)c1ccc(Nc2ncc(Br)n3ncnc23)cc1
O=C(NCc1cccnc1)c1ccc(Nc2ncc(Br)n3ncnc23)cc1
null
null
CN(C)C=O
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(NCc1cccnc1)c1ccc(Nc2nccn3ncnc23)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[#7;a:6]:[c:7]:[c:8]-[C:9]-[NH2;D1;+0:10]>>[#7;a:6]:[c:7]:[c:8]-[C:9]-[NH;D2;+0:10]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
82.3
[{"value": 82.0, "product": "BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C(=O)NCC=1C=NC=CC1)C=C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 82.3, "product": "BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C(=O)NCC=1C=NC=CC1)C=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 4-(5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-ylamino)-benzoic acid (0.230 g, 0.69 mmol), 3-hydroxybenzotriazole (0.103 g, 0.76 mmol), 1-ethyl-3-(3′-dimethylaminopropyl)carbodiimide hydrate (0.146 g, 0.76 mmol) in DMF (5 mL) and 3-picolylamine (0.077 mL, 0.76 mmol) is stirred at room temperature for 21 hours...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccncc1.c1ccccc1.c1cn2ncnc2cn1
HO-
CN(C)C=O
null
null
NCc1cccnc1.O=C(O)c1ccc(Nc2ncc(Br)n3ncnc23)cc1>CN(C)C=O>O=C(NCc1cccnc1)c1ccc(Nc2ncc(Br)n3ncnc23)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f373c043f7f84a34a628cd9ded59a339
CC1(C)OB(c2cn[nH]c2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1.O=C(NCc1cccnc1)c1ccc(Nc2ncc(Br)n3ncnc23)cc1>>N.O=C(NCc1cccnc1)c1ccc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)cc1
CC1(OB(OC1(C)C)C=1C=NNC1)C.CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2.BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C(=O)NCC=1C=NC=CC1)C=C2>>N.N1N=CC(=C1)C1=CN=C(C=2N1N=CN2)NC2=CC=C(C(=O)NCC=1C=NC=CC1)C=C2
CC1(C)OB([c:21]2[cH:22][n:23][nH:24][cH:25]2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(=O)[NH2:1])c4)n4ncnc34)cc2)CC1.Br[c:20]1[cH:19][n:18][c:17]([NH:16][c:15]2[cH:14][cH:13][c:12]([C:3](=[O:2])[NH:4][CH2:5][c:6]3[cH:7][cH:8][cH:9][n:10][cH:11]3)[cH:32][cH:31]2)[c:30]2[n:26]1[n:27][cH:28][n:29]2>>[NH3:1].[O:2]=[C:3]([NH:4]...
CC1(C)OB(c2cn[nH]c2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1.O=C(NCc1cccnc1)c1ccc(Nc2ncc(Br)n3ncnc23)cc1
N.O=C(NCc1cccnc1)c1ccc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)cc1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O1CCOCC1.C(=O)([O-])[O-].[K+].[K+]
C-C Coupling
OtherReaction
5450a2db6e7305c45383870e931e62f9935b44015cf383067240af8b2a416783
96e5f3628c1bd4659dd3e9821904115decf673d0e8e42bb7900b7f521b084c51
O=C(NCc1cccnc1)c1ccc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1.C-C1(-C)-O-B(-[c;H0;D3;+0:10]2:[c:11]:[#7;a:12]:[#7;a:13]:[c:14]:2)-O-C-1(-C)-C.C-N1-C-C-N(-c2:c:c:c(-N-c3:n:c:c(-c4:c:s:c(-C(=O)-[NH2;D1;+0:15]):c:4):n4:n:c:n:c:3:4):c:c:2)-C-C-1>>[#7;a:3]1:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]...
20
[{"value": 20.0, "product": "N1N=CC(=C1)C1=CN=C(C=2N1N=CN2)NC2=CC=C(C(=O)NCC=1C=NC=CC1)C=C2", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound may be prepared using methods as described for Compound 6, step 4 using 4-(5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-ylamino)-N-pyridin-3-ylmethyl-benzamide (100 mg, 0.24 mmol), 4-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-1H-pyrazole (93 mg, 0.48 mmol) and Pd(PPh3)4 (70 mg, 0.06 mmol) in 1.5M K2CO3 (aq...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amide.Secondary amine.Tertiary amine.Tertiary amine.Boronic ester
null
B1OCCO1.c1cn[nH]c1.C1CNCCN1.c1ccccc1.c1ccsc1.c1cn2ncnc2cn1.c1cn2ncnc2cn1
c1cn[nH]c1.c1cn2ncnc2cn1
c1ccncc1.c1ccccc1.c1cn[nH]c1.c1cn2ncnc2cn1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1.C(=O)([O-])[O-].[K+].[K+]
null
null
CC1(C)OB(c2cn[nH]c2)OC1(C)C.CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1.O=C(NCc1cccnc1)c1ccc(Nc2ncc(Br)n3ncnc23)cc1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1.C(=O)([O-])[O-...
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-21b1c2adf0644a34b21ca76c607e94a5
CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1.COc1cc(B(O)O)ccn1.O=C(NCc1cccnc1)c1ccc(Nc2ncc(Br)n3ncnc23)cc1>>COc1cc(-c2cnc(Nc3ccc(C(=O)NCc4cccnc4)cc3)c3ncnn23)ccn1.N
COC1=NC=CC(=C1)B(O)O.CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2.BrC1=CN=C(C=2N1N=CN2)NC2=CC=C(C(=O)NCC=1C=NC=CC1)C=C2>>N.COC1=NC=CC(=C1)C1=CN=C(C=2N1N=CN2)NC2=CC=C(C(=O)NCC=1C=NC=CC1)C=C2
CN1CCN(c2ccc(Nc3ncc(-c4csc(C(=O)[NH2:35])c4)n4ncnc34)cc2)CC1.OB(O)[c:5]1[cH:4][c:3]([O:2][CH3:1])[n:34][cH:33][cH:32]1.Br[c:6]1[cH:7][n:8][c:9]([NH:10][c:11]2[cH:12][cH:13][c:14]([C:15](=[O:16])[NH:17][CH2:18][c:19]3[cH:20][cH:21][cH:22][n:23][cH:24]3)[cH:25][cH:26]2)[c:27]2[n:28][cH:29][n:30][n:31]12>>[CH3:1][O:2][c:3...
CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1.COc1cc(B(O)O)ccn1.O=C(NCc1cccnc1)c1ccc(Nc2ncc(Br)n3ncnc23)cc1
COc1cc(-c2cnc(Nc3ccc(C(=O)NCc4cccnc4)cc3)c3ncnn23)ccn1.N
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O1CCOCC1.C(=O)([O-])[O-].[K+].[K+]
C-C Coupling
OtherReaction
41d4aa0ca986d610e9fc08a0f4c103dba42089333936aa6db5645b06538ea4c0
e56c7214f97d6930a188bbe94b3feccb44f2b9c6a54832ba0c9cbf78acce3e55
O=C(NCc1cccnc1)c1ccc(Nc2ncc(-c3ccncc3)n3ncnc23)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1.C-N1-C-C-N(-c2:c:c:c(-N-c3:n:c:c(-c4:c:s:c(-C(=O)-[NH2;D1;+0:10]):c:4):n4:n:c:n:c:3:4):c:c:2)-C-C-1.O-B(-O)-[c;H0;D3;+0:11]1:[c:12]:[c:13]:[#7;a:14]:[c:15](-[#8:16]):[c:17]:1>>[#8:16]-[c:15]1:[#7;a:14]:[c:13]:[c:12]:[c;H0;D3;+0:11](-[c;...
73
[{"value": 73.0, "product": "COC1=NC=CC(=C1)C1=CN=C(C=2N1N=CN2)NC2=CC=C(C(=O)NCC=1C=NC=CC1)C=C2", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This compound may be prepared using methods as described for Compound 6, step 4 using 4-(5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-ylamino)-N-pyridin-3-ylmethyl-benzamide (120 mg, 0.28 mmol), 2-methoxypyridine-4-boronic acid (87 mg, 0.57 mmol) and Pd(PPh3)4 (81 mg, 0.07 mmol) in 1.5M K2CO3 (aq) (1.6 mL) and dioxane (2.9 ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amide.Secondary amine.Tertiary amine.Tertiary amine.Boronic acid
null
C1CNCCN1.c1ccccc1.c1ccsc1.c1cn2ncnc2cn1.c1ccncc1.c1cn2ncnc2cn1
c1ccncc1.c1cn2ncnc2cn1
c1ccncc1.c1ccccc1.c1ccncc1.c1cn2ncnc2cn1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1.C(=O)([O-])[O-].[K+].[K+]
null
null
CN1CCN(c2ccc(Nc3ncc(-c4csc(C(N)=O)c4)n4ncnc34)cc2)CC1.COc1cc(B(O)O)ccn1.O=C(NCc1cccnc1)c1ccc(Nc2ncc(Br)n3ncnc23)cc1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1.C(=O)([O-])[O-].[K+].[K+...
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c2f81362810d41deb825d38a2fa6e642
COc1cc(-c2cnc(Nc3ccc(C(=O)NCc4cccnc4)cc3)c3ncnn23)ccn1>>O=C(NCc1cccnc1)c1ccc(Nc2ncc(-c3cc[nH]c(=O)c3)n3ncnc23)cc1
COC1=NC=CC(=C1)C1=CN=C(C=2N1N=CN2)NC2=CC=C(C(=O)NCC=1C=NC=CC1)C=C2.Cl.[NH+]1=CC=CC=C1>>O=C1NC=CC(=C1)C1=CN=C(C=2N1N=CN2)NC2=CC=C(C(=O)NCC=1C=NC=CC1)C=C2
C[O:25][c:24]1[n:23][cH:22][cH:21][c:20](-[c:19]2[cH:18][n:17][c:16]([NH:15][c:14]3[cH:13][cH:12][c:11]([C:2](=[O:1])[NH:3][CH2:4][c:5]4[cH:6][cH:7][cH:8][n:9][cH:10]4)[cH:33][cH:32]3)[c:31]3[n:27]2[n:28][cH:29][n:30]3)[cH:26]1>>[O:1]=[C:2]([NH:3][CH2:4][c:5]1[cH:6][cH:7][cH:8][n:9][cH:10]1)[c:11]1[cH:12][cH:13][c:14](...
COc1cc(-c2cnc(Nc3ccc(C(=O)NCc4cccnc4)cc3)c3ncnn23)ccn1
O=C(NCc1cccnc1)c1ccc(Nc2ncc(-c3cc[nH]c(=O)c3)n3ncnc23)cc1
null
null
O
Miscellaneous
OtherReaction
fb5da40428a7272a59dd461a4f5e161a7614b101c1a367e77b5ddd5b70c77e0d
291cad8b6dfbbd2c823b5c9d45efc37a166dc3454a9f151ac48cb357f4bc155f
O=C(NCc1cccnc1)c1ccc(Nc2ncc(-c3cc[nH]c(=O)c3)n3ncnc23)cc1
C-[O;H0;D2;+0:1]-[c;H0;D3;+0:2]1:[c:3]:[c:4]:[c:5]:[c:6]:[n;H0;D2;+0:7]:1>>[O;H0;D1;+0:1]=[c;H0;D3;+0:2]1:[c:3]:[c:4]:[c:5]:[c:6]:[nH;D2;+0:7]:1
49
[{"value": 49.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
150
CELSIUS
null
null
A mixture of 4-[5-(2-methoxy-pyridin-4-yl)-[1,2,4]triazolo[1,5-a]pyrazin-8-ylamino]-N-pyridin-3-ylmethyl-benzamide (71.5 mg, 0.16 mmol) and pyridinium hydrochloride (91 mg, 0.79 mmol) in water (0.5 mL) in a sealed tube is heated at 150° C. for 25 minutes. After this time the solvent is removed in vacuo. The residue is ...
10.6084/m9.figshare.5104873.v1
null
Ether
null
c1ccncc1
c1ccncc1
c1ccncc1.c1ccccc1.c1ccncc1.c1cn2ncnc2cn1
Other
O
150
null
COc1cc(-c2cnc(Nc3ccc(C(=O)NCc4cccnc4)cc3)c3ncnn23)ccn1>O>O=C(NCc1cccnc1)c1ccc(Nc2ncc(-c3cc[nH]c(=O)c3)n3ncnc23)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-43a1ea37067d45fc96a9ae3ea13df240
COc1cc([N+](=O)[O-])ccc1C(=O)O.Cc1ccc(CN)cn1>>COc1cc([N+](=O)[O-])ccc1C(=O)NCc1ccc(C)nc1
CC1=CC=C(C=N1)CN.CN1CCOCC1.CN(C)C(=[N+](C)C)ON1C2=C(C=CC=C2)N=N1.[B-](F)(F)(F)F.COC1=C(C(=O)O)C=CC(=C1)[N+](=O)[O-]>>COC1=C(C(=O)NCC=2C=NC(=CC2)C)C=CC(=C1)[N+](=O)[O-]
O[C:12]([c:11]1[c:3]([O:2][CH3:1])[cH:4][c:5]([N+:6](=[O:7])[O-:8])[cH:9][cH:10]1)=[O:13].[NH2:14][CH2:15][c:16]1[cH:17][cH:18][c:19]([CH3:20])[n:21][cH:22]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]([N+:6](=[O:7])[O-:8])[cH:9][cH:10][c:11]1[C:12](=[O:13])[NH:14][CH2:15][c:16]1[cH:17][cH:18][c:19]([CH3:20])[n:21][cH:22]1
COc1cc([N+](=O)[O-])ccc1C(=O)O.Cc1ccc(CN)cn1
COc1cc([N+](=O)[O-])ccc1C(=O)NCc1ccc(C)nc1
null
null
CN(C)C=O.C(Cl)Cl
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(NCc1cccnc1)c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[#7;a:6]:[c:7]:[c:8]-[C:9]-[NH2;D1;+0:10]>>[#7;a:6]:[c:7]:[c:8]-[C:9]-[NH;D2;+0:10]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
null
[]
null
null
30
MINUTE
2-Methoxy-4-nitrobenzoic acid (293 mg, 1.49 mmol) is dissolved in DMF (2 mL) and 4-methylmorpholine (220 μL, 3.0 mmol) and TBTU (1.79 g, 1.7 mmol) are added. The mixture is stirred at rt for 30 min and C-(6-methylpyridin-3-yl)methylamine (400 mg, 3.27 mmol) is added. Stirring is continued at rt for 12 h. DCM (10 mL) is...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccncc1
HO-
CN(C)C=O.C(Cl)Cl
null
0.5
COc1cc([N+](=O)[O-])ccc1C(=O)O.Cc1ccc(CN)cn1>CN(C)C=O.C(Cl)Cl>COc1cc([N+](=O)[O-])ccc1C(=O)NCc1ccc(C)nc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e09abf6fa88547ee8d2f16872d8b2a14
COc1cc([N+](=O)[O-])ccc1C(=O)NCc1ccc(C)nc1>>COc1cc(N)ccc1C(=O)NCc1ccc(C)nc1
COC1=C(C(=O)NCC=2C=NC(=CC2)C)C=CC(=C1)[N+](=O)[O-].C(=O)[O-].[NH4+]>>NC1=CC(=C(C(=O)NCC=2C=NC(=CC2)C)C=C1)OC
O=[N+:6]([O-])[c:5]1[cH:4][c:3]([O:2][CH3:1])[c:9]([C:10](=[O:11])[NH:12][CH2:13][c:14]2[cH:15][cH:16][c:17]([CH3:18])[n:19][cH:20]2)[cH:8][cH:7]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]([NH2:6])[cH:7][cH:8][c:9]1[C:10](=[O:11])[NH:12][CH2:13][c:14]1[cH:15][cH:16][c:17]([CH3:18])[n:19][cH:20]1
COc1cc([N+](=O)[O-])ccc1C(=O)NCc1ccc(C)nc1
COc1cc(N)ccc1C(=O)NCc1ccc(C)nc1
null
[Pd]
CCO.CCOC(=O)C
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
O=C(NCc1cccnc1)c1ccccc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
A solution of 2-methoxy-N-(6-methylpyridin-3-yl)methyl-4-nitrobenzamide (448 mg, 1.49 mmol) in EtOH and EtOAc (8 mL each) is stirred and ammonium formate (375 mg, 6 mmol) and 10% Pd/C (100 mg) are added. The mixture is heated at reflux for 20 min, cooled, filtered through celite, the solid is washed with EtOH and the c...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1.c1ccncc1
Other
[Pd].CCO.CCOC(=O)C
null
null
COc1cc([N+](=O)[O-])ccc1C(=O)NCc1ccc(C)nc1>[Pd].CCO.CCOC(=O)C>COc1cc(N)ccc1C(=O)NCc1ccc(C)nc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3e583b69311444e6ac7f180eec252c3a
Brc1ncc(Br)n2ncnc12.COc1cc(N)ccc1C(=O)NCc1ccc(C)nc1>>Cc1ccc(CNC(=O)c2ccc(Nc3ncc(Br)n4ncnc34)cc2O)cn1
BrC1=CN=C(C=2N1N=CN2)Br.NC1=CC(=C(C(=O)NCC=2C=NC(=CC2)C)C=C1)OC.C(=O)(O)[O-].[Na+].Br>>BrC1=CN=C(C=2N1N=CN2)NC2=CC(=C(C(=O)NCC=1C=NC(=CC1)C)C=C2)O
Br[c:15]1[n:16][cH:17][c:18]([Br:19])[n:20]2[n:21][cH:22][n:23][c:24]12.C[O:27][c:26]1[c:10]([C:8]([NH:7][CH2:6][c:5]2[cH:4][cH:3][c:2]([CH3:1])[n:29][cH:28]2)=[O:9])[cH:11][cH:12][c:13]([NH2:14])[cH:25]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([CH2:6][NH:7][C:8](=[O:9])[c:10]2[cH:11][cH:12][c:13]([NH:14][c:15]3[n:16][cH:17][c...
Brc1ncc(Br)n2ncnc12.COc1cc(N)ccc1C(=O)NCc1ccc(C)nc1
Cc1ccc(CNC(=O)c2ccc(Nc3ncc(Br)n4ncnc34)cc2O)cn1
null
null
O.CC(C)O
Heteroatom Alkylation and Arylation
OtherReaction
e8830d2dc159e2698fd6973d85ee5c0f5af45e99dfb394e286d23433deb9893b
6b24500fd64e6aa86066d0cc793af94111bb9f672d4a0bca714da9676cbd049d
O=C(NCc1cccnc1)c1ccc(Nc2nccn3ncnc23)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:1.C-[O;H0;D2;+0:10]-[c:11](:[c:12]-[C:13](-[#7:14])=[O;D1;H0:15]):[c:16]:[c:17](-[NH2;D1;+0:18]):[c:19]>>[#7:14]-[C:13](=[O;D1;H0:15])-[c:12]:[c:11](-[OH;D1;+0:10]):[c:16]:[c:17](-[NH;D2;+0:18]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5...
null
[]
null
null
null
null
5,8-Dibromo-[1,2,4]triazolo[1,5-a]pyrazine (285 mg, 1.03 mmol) and 4-amino-2-methoxy-N-[(6-methylpyridin-3-yl)methyl]benzamide (280 mg, 1.03 mmol) are stirred in iPrOH (5 mL) and HBr (48% aq., 380 μL) is added. The mixture is heated at reflux for 24 hours. The cooled suspension is poured into NaHCO3 (sat. aq., 25 mL) a...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ether.Primary amine
Aromatic alcohol.Secondary amine
c1cn2ncnc2cn1
c1cn2ncnc2cn1
c1ccncc1.c1ccccc1.c1cn2ncnc2cn1
HBr
O.CC(C)O
null
null
Brc1ncc(Br)n2ncnc12.COc1cc(N)ccc1C(=O)NCc1ccc(C)nc1>O.CC(C)O>Cc1ccc(CNC(=O)c2ccc(Nc3ncc(Br)n4ncnc34)cc2O)cn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a4ed936621f141269e1e5d0a8eea41f3
CO.Cc1ccc(CNC(=O)c2ccc(Nc3ncc(Br)n4ncnc34)cc2O)cn1.OB(O)c1cn[nH]c1>>COc1cc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)ccc1C(=O)NCc1ccc(C)nc1
S(=O)(=O)(C)O.CO.N1N=CC(=C1)B(O)O.BrC1=CN=C(C=2N1N=CN2)NC2=CC(=C(C(=O)NCC=1C=NC(=CC1)C)C=C2)O.C(=O)([O-])[O-].[K+].[K+]>>COC1=C(C(=O)NCC=2C=NC(=CC2)C)C=CC(=C1)NC=1C=2N(C(=CN1)C=1C=NNC1)N=CN2
O[CH3:1].Br[c:10]1[cH:9][n:8][c:7]([NH:6][c:5]2[cH:4][c:3]([OH:2])[c:23]([C:24](=[O:25])[NH:26][CH2:27][c:28]3[cH:29][cH:30][c:31]([CH3:32])[n:33][cH:34]3)[cH:22][cH:21]2)[c:20]2[n:16]1[n:17][cH:18][n:19]2.OB(O)[c:11]1[cH:12][n:13][nH:14][cH:15]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]([NH:6][c:7]2[n:8][cH:9][c:10](-[c:11]3[cH:...
CO.Cc1ccc(CNC(=O)c2ccc(Nc3ncc(Br)n4ncnc34)cc2O)cn1.OB(O)c1cn[nH]c1
COc1cc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)ccc1C(=O)NCc1ccc(C)nc1
null
null
CO.C(Cl)Cl
Heteroatom Alkylation and Arylation
OtherReaction
8295d8dececbac203070bd99fb61929320bf39ddf2b72d768876bc703cc58d7b
f5eba816ddabe8705e2883ca2473fe0e738ffcc54103fca4c8d83d6d2a00241c
O=C(NCc1cccnc1)c1ccc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1.[#7:10]-[C:11](=[O;D1;H0:12])-[c:13]:[c:14](-[OH;D1;+0:15]):[c:16].O-B(-O)-[c;H0;D3;+0:17]1:[c:18]:[#7;a:19]:[#7;a:20]:[c:21]:1.O-[CH3;D1;+0:22]>>[#7;a:19]1:[#7;a:20]:[c:21]:[c;H0;D3;+0:17](-[c;H0;D3;+0:1]2:[c:2]:[#7;a:3]:[c:4]:[c:5]3:[...
null
[]
null
null
30
SECOND
Pyrazole-4-boronic acid (19 mg, 0.17 mmol), 4-(5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-ylamino)-2-hydroxy-N-[(6-methyl-pyridin-3-yl)methyl]benzamide (40 mg, 0.085 mmol), K2CO3 (24 mg, 0.17 mmol) and Pd(dppf)Cl2CH2Cl2 (4 mg, 0.005 mmol) are weighed into a sealable tube. The tube is flushed with nitrogen and dioxane-wate...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol.Boronic acid.Methanol
Ether
c1cn2ncnc2cn1.c1cn[nH]c1
c1cn[nH]c1.c1cn2ncnc2cn1
c1ccccc1.c1cn[nH]c1.c1cn2ncnc2cn1.c1ccncc1
HBr.B
CO.C(Cl)Cl
null
0.008333
CO.Cc1ccc(CNC(=O)c2ccc(Nc3ncc(Br)n4ncnc34)cc2O)cn1.OB(O)c1cn[nH]c1>CO.C(Cl)Cl>COc1cc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)ccc1C(=O)NCc1ccc(C)nc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-873f23cfc9084ae2bf7e9ba4c604e5c3
COc1cc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)ccc1C(=O)NCc1ccc(C)nc1.NCc1ccccc1>>COc1cc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)ccc1C(=O)NCc1ccccc1
COC1=C(C(=O)NCC=2C=NC(=CC2)C)C=CC(=C1)NC=1C=2N(C(=CN1)C=1C=NNC1)N=CN2.C(C1=CC=CC=C1)N>>C(C1=CC=CC=C1)NC(C1=C(C=C(C=C1)NC=1C=2N(C(=CN1)C=1C=NNC1)N=CN2)OC)=O
Cc1cc[c:28]([CH2:27][NH:26][C:24]([c:23]2[c:3]([O:2][CH3:1])[cH:4][c:5]([NH:6][c:7]3[n:8][cH:9][c:10](-[c:11]4[cH:12][n:13][nH:14][cH:15]4)[n:16]4[n:17][cH:18][n:19][c:20]34)[cH:21][cH:22]2)=[O:25])[cH:33]n1.NCc1c[cH:32][cH:31][cH:30][cH:29]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]([NH:6][c:7]2[n:8][cH:9][c:10](-[c:11]3[cH:12][...
COc1cc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)ccc1C(=O)NCc1ccc(C)nc1.NCc1ccccc1
COc1cc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)ccc1C(=O)NCc1ccccc1
null
null
null
Miscellaneous
OtherReaction
d1e52c14e3c13261c493bba43efa0cd5dea570c8557c0c45e5137a6ced83376d
74f861e099b6420f2f6d4f3094b402eaca1d0baec018283dff42a39bacc23c31
O=C(NCc1ccccc1)c1ccc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)cc1
C-c1:c:c:[c;H0;D3;+0:1](-[C:2]-[#7:3]-[C:4]=[O;D1;H0:5]):[cH;D2;+0:6]:n:1.N-C-c1:[cH;D2;+0:7]:[c:8]:[c:9]:[cH;D2;+0:10]:c:1>>[O;D1;H0:5]=[C:4]-[#7:3]-[C:2]-[c;H0;D3;+0:1]1:[cH;D2;+0:7]:[c:8]:[c:9]:[cH;D2;+0:10]:[cH;D2;+0:6]:1
null
[]
null
null
null
null
This compound may be prepared using the methods described for Compound 120, using benzylamine in step 1. LCMS: Rt 1.62 min (100%) m/z (ESI) 440 (M+H)+. Conditions: See reaction.notes.procedure_details. Workup: This compound may be prepared
10.6084/m9.figshare.5104873.v1
null
Primary amine
null
c1ccncc1.c1ccccc1
c1ccccc1
c1ccccc1.c1cn[nH]c1.c1cn2ncnc2cn1.c1ccccc1
Other
null
null
null
COc1cc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)ccc1C(=O)NCc1ccc(C)nc1.NCc1ccccc1>>COc1cc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)ccc1C(=O)NCc1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5a9e8cf340204f16a39d32d54c680c26
Brc1ncc(Br)n2ncnc12.CCOC(=O)c1cccc(N)c1>>CCOC(=O)c1cccc(Nc2ncc(Br)n3ncnc23)c1
BrC1=CN=C(C=2N1N=CN2)Br.NC=1C=C(C(=O)OCC)C=CC1.Br>>C(C)OC(C1=CC(=CC=C1)NC=1C=2N(C(=CN1)Br)N=CN2)=O
Br[c:12]1[n:13][cH:14][c:15]([Br:16])[n:17]2[n:18][cH:19][n:20][c:21]12.[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][cH:9][c:10]([NH2:11])[cH:22]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][cH:9][c:10]([NH:11][c:12]2[n:13][cH:14][c:15]([Br:16])[n:17]3[n:18][cH:19][n:20][c:21]23)[cH:22]1
Brc1ncc(Br)n2ncnc12.CCOC(=O)c1cccc(N)c1
CCOC(=O)c1cccc(Nc2ncc(Br)n3ncnc23)c1
null
null
CC(C)O
Heteroatom Alkylation and Arylation
N-arylation (Buchwald-Hartwig/Ullmann-Goldberg)
aecfb0ede2c5d7901fea69101287828edf21f7a6e48b6ff83fe43de0688f1ef1
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(Nc2nccn3ncnc23)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:1.[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[c:12]:[c:11](-[NH;D2;+0:10]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:1):[c:13]
98
[{"value": 98.0, "product": "C(C)OC(C1=CC(=CC=C1)NC=1C=2N(C(=CN1)Br)N=CN2)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
85
CELSIUS
null
null
5,8-Dibromo-[1,2,4]triazolo[1,5-a]pyrazine (1.39 g, 5.00 mmol) and ethyl 3-aminobenzoate (0.93 g, 5.60 mmol) are stirred in iPrOH (10 mL) and HBr (48% aq., 1.14 mL, 10 mmol) is added. The mixture is heated at 85° C. for 4 h and then cooled to rt and quenched with NaHCO3 (sat. aq., 25 mL). The resulting suspension is co...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1cn2ncnc2cn1
c1cn2ncnc2cn1
c1ccccc1.c1cn2ncnc2cn1
HBr
CC(C)O
85
null
Brc1ncc(Br)n2ncnc12.CCOC(=O)c1cccc(N)c1>CC(C)O>CCOC(=O)c1cccc(Nc2ncc(Br)n3ncnc23)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e25402d3b56c47beafa2a07d55f06a9a
CC(C)(C)OC(=O)OC(=O)OC(C)(C)C.CCOC(=O)c1cccc(Nc2ncc(Br)n3ncnc23)c1>>CCOC(=O)c1cccc(N(C(=O)OC(C)(C)C)c2ncc(Br)n3ncnc23)c1
C(C)OC(C1=CC(=CC=C1)NC=1C=2N(C(=CN1)Br)N=CN2)=O.O(C(=O)OC(C)(C)C)C(=O)OC(C)(C)C>>C(C)OC(C1=CC(=CC=C1)N(C(=O)OC(C)(C)C)C=1C=2N(C(=CN1)Br)N=CN2)=O
CC(C)(C)OC(=O)O[C:12](=[O:13])[O:14][C:15]([CH3:16])([CH3:17])[CH3:18].[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][cH:9][c:10]([NH:11][c:19]2[n:20][cH:21][c:22]([Br:23])[n:24]3[n:25][cH:26][n:27][c:28]23)[cH:29]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][cH:9][c:10]([N:11]([C:12](=[O:13])[O:14][C:15]([...
CC(C)(C)OC(=O)OC(=O)OC(C)(C)C.CCOC(=O)c1cccc(Nc2ncc(Br)n3ncnc23)c1
CCOC(=O)c1cccc(N(C(=O)OC(C)(C)C)c2ncc(Br)n3ncnc23)c1
null
CN(C)C=1C=CN=CC1
C(Cl)Cl
Protection
Boc amine protection with Boc anhydride
179c37a0cfe150b9a322c3349c8b39605fd97b04b0abb3f5b3c182be0494cd4b
7c9d9ba915c29b1020a278f50f3c8f9cc1fd09ebab5bff22f0c1b047d4ae169a
c1ccc(Nc2nccn3ncnc23)cc1
C-C(-C)(-C)-O-C(=O)-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C:4](-[C;D1;H3:5])(-[C;D1;H3:6])-[C;D1;H3:7].[c:8]:[c:9](-[NH;D2;+0:10]-[c:11]1:[#7;a:12]:[c:13]:[c:14]:[#7;a:15]2:[#7;a:16]:[c:17]:[#7;a:18]:[c:19]:2:1):[c:20]>>[C;D1;H3:5]-[C:4](-[C;D1;H3:6])(-[C;D1;H3:7])-[#8:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[N;H0;D3;+0:10](-...
81.1
[{"value": 81.1, "product": "C(C)OC(C1=CC(=CC=C1)N(C(=O)OC(C)(C)C)C=1C=2N(C(=CN1)Br)N=CN2)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
A solution of 3-(5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-ylamino)benzoic acid ethyl ester (1.79 g, 4.93 mmol) in DCM (20 mL) is stirred under N2 at rt and BOC2O (1.34 g, 6.16 mmol) and DMAP (0.30 g, 2.46 mmol) are added. Stirring is continued for 2 h, when LCMS indicates complete conversion of the starting material. Th...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Carbonic Ester.Carbonic Ester.Secondary amine.Boc.Boc
Carbamic ester
null
null
c1ccccc1.c1cn2ncnc2cn1
HO-
CN(C)C=1C=CN=CC1.C(Cl)Cl
null
2
CC(C)(C)OC(=O)OC(=O)OC(C)(C)C.CCOC(=O)c1cccc(Nc2ncc(Br)n3ncnc23)c1>CN(C)C=1C=CN=CC1.C(Cl)Cl>CCOC(=O)c1cccc(N(C(=O)OC(C)(C)C)c2ncc(Br)n3ncnc23)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-330b23e505d84149a2cbb0351f283546
CC1(C)OB(c2cn[nH]c2)OC1(C)C.CCOC(=O)c1cccc(N(C(=O)OC(C)(C)C)c2ncc(Br)n3ncnc23)c1>>CCOC(=O)c1cccc(N(C(=O)OC(C)(C)C)c2ncc(-c3cn[nH]c3)n3ncnc23)c1
C(C)OC(C1=CC(=CC=C1)N(C(=O)OC(C)(C)C)C=1C=2N(C(=CN1)Br)N=CN2)=O.CC1(OB(OC1(C)C)C=1C=NNC1)C.C(=O)([O-])[O-].[K+].[K+]>>C(C)OC(C1=CC(=CC=C1)N(C=1C=2N(C(=CN1)C=1C=NNC1)N=CN2)C(=O)OC(C)(C)C)=O
CC1(C)OB([c:23]2[cH:24][n:25][nH:26][cH:27]2)OC1(C)C.Br[c:22]1[cH:21][n:20][c:19]([N:11]([c:10]2[cH:9][cH:8][cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[cH:33]2)[C:12](=[O:13])[O:14][C:15]([CH3:16])([CH3:17])[CH3:18])[c:32]2[n:28]1[n:29][cH:30][n:31]2>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][cH:9][c:10]([N:...
CC1(C)OB(c2cn[nH]c2)OC1(C)C.CCOC(=O)c1cccc(N(C(=O)OC(C)(C)C)c2ncc(Br)n3ncnc23)c1
CCOC(=O)c1cccc(N(C(=O)OC(C)(C)C)c2ncc(-c3cn[nH]c3)n3ncnc23)c1
null
null
O1CCOCC1.O
C-C Coupling
Suzuki coupling with boronic esters
3b077e58a8068174133a7eecad35957570f9290725408c31a955826b02d2e470
b42efb3b6a7742d5af594c6a3031e487327e58e9f8c2f428ee68996c98377910
c1ccc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1.C-C1(-C)-O-B(-[c;H0;D3;+0:10]2:[c:11]:[#7;a:12]:[#7;a:13]:[c:14]:2)-O-C-1(-C)-C>>[#7;a:3]1:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:[c;H0;D3;+0:1](-[c;H0;D3;+0:10]2:[c:11]:[#7;a:12]:[#7;a:13]:[c:14]:2):[c:2]:1
108.6
[{"value": 100.0, "product": "C(C)OC(C1=CC(=CC=C1)N(C=1C=2N(C(=CN1)C=1C=NNC1)N=CN2)C(=O)OC(C)(C)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 108.6, "product": "C(C)OC(C1=CC(=CC=C1)N(C=1C=2N(C(=CN1)C=1C=NNC1)N=CN2)C(=O)OC(C)(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
115
CELSIUS
null
null
Nitrogen is bubbled through a mixture of 3-[(5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-yl)-tert-butoxycarbonyl-amino]benzoic acid ethyl ester (0.58 g, 1.25 mmol), 4-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-1H-pyrazole (0.49 g, 2.50 mmol), K2CO3 (0.35 g, 2.50 mmol) and Pd(dppf)Cl2DCM (102 mg, 0.125 mmol) in dioxane ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic ester
null
B1OCCO1.c1cn[nH]c1.c1cn2ncnc2cn1
c1cn[nH]c1.c1cn2ncnc2cn1
c1ccccc1.c1cn[nH]c1.c1cn2ncnc2cn1
HBr.B
O1CCOCC1.O
115
null
CC1(C)OB(c2cn[nH]c2)OC1(C)C.CCOC(=O)c1cccc(N(C(=O)OC(C)(C)C)c2ncc(Br)n3ncnc23)c1>O1CCOCC1.O>CCOC(=O)c1cccc(N(C(=O)OC(C)(C)C)c2ncc(-c3cn[nH]c3)n3ncnc23)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-828742442cf1402b967da9c94c959a02
CC(C)(C)OC(=O)N(c1cccc(C(=O)O)c1)c1ncc(-c2cn[nH]c2)n2ncnc12.CCN>>CCNC(=O)c1cccc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)c1
C(C)(C)(C)OC(=O)N(C=1C=C(C(=O)O)C=CC1)C=1C=2N(C(=CN1)C=1C=NNC1)N=CN2.C(C)N.Cl.C1CCN(C1)[P+](N2CCCC2)(N3CCCC3)ON4C5=C(C=CC=C5)N=N4.F[P-](F)(F)(F)(F)F>>C(C)NC(C1=CC(=CC=C1)NC=1C=2N(C(=CN1)C=1C=NNC1)N=CN2)=O
CC(C)(C)OC(=O)[N:11]([c:10]1[cH:9][cH:8][cH:7][c:6]([C:4](O)=[O:5])[cH:26]1)[c:12]1[n:13][cH:14][c:15](-[c:16]2[cH:17][n:18][nH:19][cH:20]2)[n:21]2[n:22][cH:23][n:24][c:25]12.[CH3:1][CH2:2][NH2:3]>>[CH3:1][CH2:2][NH:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][cH:9][c:10]([NH:11][c:12]2[n:13][cH:14][c:15](-[c:16]3[cH:17][n:18][nH...
CC(C)(C)OC(=O)N(c1cccc(C(=O)O)c1)c1ncc(-c2cn[nH]c2)n2ncnc12.CCN
CCNC(=O)c1cccc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)c1
null
null
CO.CCO.C(C)N(CC)CC.CN(C)C=O
Acylation
OtherReaction
f10fdabbb25888046326b895dd209630fab45b1d73614d556710fe29012f39e4
9f74be20683ae20656a7135e9a9eaad2dfa782f75ac656d32f38d1324fe876ad
c1ccc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)cc1
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1](-[c:2](:[c:3]):[c:4]:[c:5](-[C;H0;D3;+0:6](-O)=[O;D1;H0:7]):[c:8])-[c:9]1:[#7;a:10]:[c:11]:[c:12]:[#7;a:13]2:[#7;a:14]:[c:15]:[#7;a:16]:[c:17]:2:1.[C;D1;H3:18]-[C:19]-[NH2;D1;+0:20]>>[C;D1;H3:18]-[C:19]-[NH;D2;+0:20]-[C;H0;D3;+0:6](=[O;D1;H0:7])-[c:5](:[c:8]):[c:4]:[c:2](-[NH;D2;+0:1]...
20.1
[{"value": 20.1, "product": "C(C)NC(C1=CC(=CC=C1)NC=1C=2N(C(=CN1)C=1C=NNC1)N=CN2)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
3-{tert-Butoxycarbonyl-[5-(1H-pyrazol-4-yl)-[1,2,4]triazolo[1,5-a]pyrazin-8-yl]-amino}benzoic acid (42 mg, 0.10 mmol), ethylamine (12 M aq., 42 μL, 0.50 mmol), and triethylamine (28 μL, 0.20 mmol) are stirred in DMF (0.30 mL) and PyBOP (57 mg, 0.11 mmol) is added. Stirring is continued overnight. The reaction mixture i...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Carboxylic acid.Ether.Primary amine.Boc
Secondary amide.Secondary amine
null
null
c1ccccc1.c1cn[nH]c1.c1cn2ncnc2cn1
HO-
CO.CCO.C(C)N(CC)CC.CN(C)C=O
null
8
CC(C)(C)OC(=O)N(c1cccc(C(=O)O)c1)c1ncc(-c2cn[nH]c2)n2ncnc12.CCN>CO.CCO.C(C)N(CC)CC.CN(C)C=O>CCNC(=O)c1cccc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7c7545711ee54f68bf948b0658f08455
CCNC(=O)c1cccc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)c1.NCc1ccc(O)cc1>>O=C(NCc1ccc(O)cc1)c1cccc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)c1
C(C)NC(C1=CC(=CC=C1)NC=1C=2N(C(=CN1)C=1C=NNC1)N=CN2)=O.OC1=CC=C(CN)C=C1>>OC1=CC=C(CNC(C2=CC(=CC=C2)NC=2C=3N(C(=CN2)C=2C=NNC2)N=CN3)=O)C=C1
CCN[C:2](=[O:1])[c:12]1[cH:13][cH:14][cH:15][c:16]([NH:17][c:18]2[n:19][cH:20][c:21](-[c:22]3[cH:23][n:24][nH:25][cH:26]3)[n:27]3[n:28][cH:29][n:30][c:31]23)[cH:32]1.[NH2:3][CH2:4][c:5]1[cH:6][cH:7][c:8]([OH:9])[cH:10][cH:11]1>>[O:1]=[C:2]([NH:3][CH2:4][c:5]1[cH:6][cH:7][c:8]([OH:9])[cH:10][cH:11]1)[c:12]1[cH:13][cH:14...
CCNC(=O)c1cccc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)c1.NCc1ccc(O)cc1
O=C(NCc1ccc(O)cc1)c1cccc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)c1
null
null
null
Acylation
OtherReaction
8ccec54884e2cbe7f97f6cea5ae365674b20e64bfde0c57faeea449854021acc
4accd3f274dad8ca7d44350b7d7da15181b5e5579c068528178b23416d2aea4a
O=C(NCc1ccccc1)c1cccc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)c1
C-C-N-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[NH2;D1;+0:6]-[C:7]-[c:8]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[C:7]-[c:8])-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
This compound may be prepared using methods as described for Compound 129, using 4-hydroxybenzylamine in step 5. LCMS: Rt=0.98 min (100%), m/z (ESI) 427 (M+H)+. Conditions: See reaction.notes.procedure_details. Workup: This compound may be prepared
10.6084/m9.figshare.5104873.v1
null
Secondary amide.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccccc1.c1cn[nH]c1.c1cn2ncnc2cn1
Other
null
null
null
CCNC(=O)c1cccc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)c1.NCc1ccc(O)cc1>>O=C(NCc1ccc(O)cc1)c1cccc(Nc2ncc(-c3cn[nH]c3)n3ncnc23)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-de4280073ef14b95aee133186ee3a2e6
NC(=O)c1cc(B(O)O)cs1.O=C(Cc1ccccc1)Nc1ccc(Nc2ncc(Br)n3ncnc23)cn1>>NC(=O)c1cc(-c2cnc(Nc3ccc(NC(=O)Cc4ccccc4)nc3)c3ncnn23)cs1
COC1=C(C(=O)NCC=2C=NC(=CC2)C)C=CC(=C1)NC=1C=2N(C(=CN1)C=1C=NNC1)N=CN2.BrC1=CN=C(C=2N1N=CN2)NC=2C=CC(=NC2)NC(CC2=CC=CC=C2)=O.NC(=O)C=1SC=C(C1)B(O)O>>C1(=CC=CC=C1)CC(=O)NC1=CC=C(C=N1)NC=1C=2N(C(=CN1)C=1C=C(SC1)C(=O)N)N=CN2
OB(O)[c:6]1[cH:5][c:4]([C:2]([NH2:1])=[O:3])[s:34][cH:33]1.Br[c:7]1[cH:8][n:9][c:10]([NH:11][c:12]2[cH:13][cH:14][c:15]([NH:16][C:17](=[O:18])[CH2:19][c:20]3[cH:21][cH:22][cH:23][cH:24][cH:25]3)[n:26][cH:27]2)[c:28]2[n:29][cH:30][n:31][n:32]12>>[NH2:1][C:2](=[O:3])[c:4]1[cH:5][c:6](-[c:7]2[cH:8][n:9][c:10]([NH:11][c:12...
NC(=O)c1cc(B(O)O)cs1.O=C(Cc1ccccc1)Nc1ccc(Nc2ncc(Br)n3ncnc23)cn1
NC(=O)c1cc(-c2cnc(Nc3ccc(NC(=O)Cc4ccccc4)nc3)c3ncnn23)cs1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
43d3551703d0592fc09d7e8a4fc6f079755043a628c77b3213d51db104641e47
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C(Cc1ccccc1)Nc1ccc(Nc2ncc(-c3ccsc3)n3ncnc23)cn1
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[#7;a:9]:2:1.O-B(-O)-[c;H0;D3;+0:10]1:[c:11]:[#16;a:12]:[c:13](-[C:14](-[N;D1;H2:15])=[O;D1;H0:16]):[c:17]:1>>[N;D1;H2:15]-[C:14](=[O;D1;H0:16])-[c:13]1:[#16;a:12]:[c:11]:[c;H0;D3;+0:10](-[c;H0;D3;+0:1]2:[c:2]:[#7;a:3]:[c:4]:[c:5]3:[#7;a:6]:[c:7]:[#...
null
[]
null
null
null
null
This compound may be prepared using methods as described for Compound 120, step 4, using N-[5-(5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-ylamino)-pyridin-2-yl]-2-phenylacetamide and 2-(aminocarbonyl)thiophene-4-boronic acid. LCMS: Rt 1.06 min (100%) m/z (ESI) 471 (M+H)+. Conditions: See reaction.notes.procedure_details. ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccsc1.c1cn2ncnc2cn1
c1ccsc1.c1cn2ncnc2cn1
c1ccsc1.c1ccncc1.c1ccccc1.c1cn2ncnc2cn1
HBr.B
null
null
null
NC(=O)c1cc(B(O)O)cs1.O=C(Cc1ccccc1)Nc1ccc(Nc2ncc(Br)n3ncnc23)cn1>>NC(=O)c1cc(-c2cnc(Nc3ccc(NC(=O)Cc4ccccc4)nc3)c3ncnn23)cs1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-412c6895c66746fb9d5be9457be48763
CC(C)N1CCC(c2ccc(Nc3ncc(-c4cn[nH]c4)n4ncnc34)cc2)CC1.NC(=O)CBr>>NC(=O)CN1CCC(c2ccc(Nc3ncc(-c4cn[nH]c4)n4ncnc34)cc2)CC1
C(C)(C)N1CCC(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=NNC1)N=CN2.BrCC(=O)N>>N1N=CC(=C1)C1=CN=C(C=2N1N=CN2)NC2=CC=C(C=C2)C2CCN(CC2)CC(=O)N
CC(C)[N:5]1[CH2:6][CH2:7][CH:8]([c:9]2[cH:10][cH:11][c:12]([NH:13][c:14]3[n:15][cH:16][c:17](-[c:18]4[cH:19][n:20][nH:21][cH:22]4)[n:23]4[n:24][cH:25][n:26][c:27]34)[cH:28][cH:29]2)[CH2:30][CH2:31]1.Br[CH2:4][C:2]([NH2:1])=[O:3]>>[NH2:1][C:2](=[O:3])[CH2:4][N:5]1[CH2:6][CH2:7][CH:8]([c:9]2[cH:10][cH:11][c:12]([NH:13][c...
CC(C)N1CCC(c2ccc(Nc3ncc(-c4cn[nH]c4)n4ncnc34)cc2)CC1.NC(=O)CBr
NC(=O)CN1CCC(c2ccc(Nc3ncc(-c4cn[nH]c4)n4ncnc34)cc2)CC1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
15cc3a5a9d32314b79094a0e5ab12888144a1ec35cfb2d8d6a128315fd0f10a2
b6177f1fc9b2dcf6edc7b8787c5dfef88aa31b4557820e58fa8b5889998b8498
c1nc2c(Nc3ccc(C4CCNCC4)cc3)ncc(-c3cn[nH]c3)n2n1
Br-[CH2;D2;+0:1]-[C:2](-[N;D1;H2:3])=[O;D1;H0:4].C-C(-C)-[N;H0;D3;+0:5](-[C:6]-[C:7])-[C:8]-[C:9]>>[C:7]-[C:6]-[N;H0;D3;+0:5](-[CH2;D2;+0:1]-[C:2](-[N;D1;H2:3])=[O;D1;H0:4])-[C:8]-[C:9]
null
[]
null
null
null
null
This compound may be prepared using methods as described for Compound 84, using 2-bromoacetamide in step 1. LCMS: Rt=0.81 min (100%), m/z (ESI) 418 (M+H)+. Conditions: See reaction.notes.procedure_details. Workup: This compound may be prepared
10.6084/m9.figshare.5104873.v1
null
Primary halide.Tertiary amine
Tertiary amine
C1CC[NH]CC1
C1CC[NH]CC1
C1CC[NH]CC1.c1ccccc1.c1cn[nH]c1.c1cn2ncnc2cn1
HBr
null
null
null
CC(C)N1CCC(c2ccc(Nc3ncc(-c4cn[nH]c4)n4ncnc34)cc2)CC1.NC(=O)CBr>>NC(=O)CN1CCC(c2ccc(Nc3ncc(-c4cn[nH]c4)n4ncnc34)cc2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e3efd46fcb63474ea53f3e896a9dbfb8
CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2C(F)(F)F)CC1.c1nc2c(Nc3ccc(N4CCN(CC5CC5)CC4)cc3)ncc(-c3cn[nH]c3)n2n1>>CC(C)N1CCN(c2ccc(Nc3ncc(-c4cn[nH]c4)n4ncnc34)cc2C(F)(F)F)CC1
C1(CC1)CN1CCN(CC1)C1=CC=C(C=C1)NC=1C=2N(C(=CN1)C=1C=NNC1)N=CN2.BrC1=CN=C(C=2N1N=CN2)NC2=CC(=C(C=C2)N2CCN(CC2)C(C)C)C(F)(F)F>>C(C)(C)N1CCN(CC1)C1=C(C=C(C=C1)NC=1C=2N(C(=CN1)C=1C=NNC1)N=CN2)C(F)(F)F
Brc1cnc(N[c:11]2[cH:10][cH:9][c:8]([N:7]3[CH2:6][CH2:5][N:4]([CH:2]([CH3:1])[CH3:3])[CH2:34][CH2:33]3)[c:28]([C:29]([F:30])([F:31])[F:32])[cH:27]2)c2ncnn12.c1cc([NH:12][c:13]2[n:14][cH:15][c:16](-[c:17]3[cH:18][n:19][nH:20][cH:21]3)[n:22]3[n:23][cH:24][n:25][c:26]23)ccc1N1CCN(CC2CC2)CC1>>[CH3:1][CH:2]([CH3:3])[N:4]1[CH...
CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2C(F)(F)F)CC1.c1nc2c(Nc3ccc(N4CCN(CC5CC5)CC4)cc3)ncc(-c3cn[nH]c3)n2n1
CC(C)N1CCN(c2ccc(Nc3ncc(-c4cn[nH]c4)n4ncnc34)cc2C(F)(F)F)CC1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
5ddda3b84343a55f86a0261fb38b43781f64e63aa92481f1cf27df1481179a38
7d31f47e5761ed6e1805ce0becec02c3b3cb1ec75262e81cbdbb96933cfa3652
c1nc2c(Nc3ccc(N4CCNCC4)cc3)ncc(-c3cn[nH]c3)n2n1
Br-c1:c:n:c(-N-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):c2:n:c:n:n:1:2.C1-C-C-1-C-N1-C-C-N(-c2:c:c:c(-[NH;D2;+0:6]-[c:7]3:[#7;a:8]:[c:9]:[c:10]:[#7;a:11]4:[#7;a:12]:[c:13]:[#7;a:14]:[c:15]:4:3):c:c:2)-C-C-1>>[c:5]:[c:4]:[c;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7]1:[#7;a:8]:[c:9]:[c:10]:[#7;a:11]2:[#7;a:12]:[c:13]:[#7;a:14]:[c:...
null
[]
null
null
null
null
This compound may be prepared using methods as described for Compound 46, using (5-bromo-[1,2,4]triazolo[1,5-a]pyrazin-8-yl)-[4-(4-isopropylpiperazin-1-yl)-3-trifluoromethylphenyl]amine. LCMS: Rt=0.99 (95%), m/z (ESI) 472 (M+H)+. Conditions: See reaction.notes.procedure_details. Workup: This compound may be prepared
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Secondary amine.Secondary amine.Tertiary amine.Tertiary amine
Secondary amine
c1ccccc1.c1cn2ncnc2cn1.c1ccccc1.C1CNCCN1.C1CC1
c1ccccc1
C1C[NH]CC[NH]1.c1ccccc1.c1cn[nH]c1.c1cn2ncnc2cn1
HBr
null
null
null
CC(C)N1CCN(c2ccc(Nc3ncc(Br)n4ncnc34)cc2C(F)(F)F)CC1.c1nc2c(Nc3ccc(N4CCN(CC5CC5)CC4)cc3)ncc(-c3cn[nH]c3)n2n1>>CC(C)N1CCN(c2ccc(Nc3ncc(-c4cn[nH]c4)n4ncnc34)cc2C(F)(F)F)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d6cc889528434fa396a38aa8ba73abe0
CC(C)O.O=C1c2ccccc2C(=O)C1(O)O.[NH4+]>>OC[C@H]1CNC[C@@H](O)[C@@H]1O
C(C)(C)O.O.[NH4+].[OH-].C1=CC=C2C(=C1)C(=O)C(C2=O)(O)O>>C1[C@@H]([C@H]([C@@H](CN1)O)O)CO
C[CH:2]([OH:1])[CH3:6].O=C1c2ccc[cH:4][c:3]2[C:9](=[O:10])[C:7]1(O)[OH:8].[NH4+:5]>>[OH:1][CH2:2][C@H:3]1[CH2:4][NH:5][CH2:6][C@@H:7]([OH:8])[C@@H:9]1[OH:10]
CC(C)O.O=C1c2ccccc2C(=O)C1(O)O.[NH4+]
OC[C@H]1CNC[C@@H](O)[C@@H]1O
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
e73a4ecfdecb42a1d125106a488e57a4c13823fbf77aa549c85a69c894ce7237
6501933472fecd70b0b1194b8ef7ca3a85539167470ffd6be89ccc9ea97365d3
C1CCNCC1
C-[CH;D3;+0:1](-[CH3;D1;+0:2])-[O;D1;H1:3].O-[C;H0;D4;+0:4]1(-[O;D1;H1:5])-C(=O)-c2:c:c:c:[cH;D2;+0:6]:[c;H0;D3;+0:7]:2-[C;H0;D3;+0:8]-1=[O;H0;D1;+0:9].[NH4+;D0:10]>>[O;D1;H1:3]-[CH2;D2;+0:1]-[C@H;D3;+0:7]1-[CH2;D2;+0:6]-[NH;D2;+0:10]-[CH2;D2;+0:2]-[C@@H;D3;+0:4](-[O;D1;H1:5])-[C@@H;D3;+0:8]-1-[OH;D1;+0:9]
null
[]
null
null
72
HOUR
TLC was performed on the different fractions (silica gel, isopropanol:water:NH4OH (7:2:1) and detection was via imino sugar and ninhydrin spray. Fractions testing positive with the imino-sugar sprays were analyzed to determine purity, then combined and lyophilized for 72 hours. Conditions: See reaction.notes.procedure_...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ketone.Secondary alcohol.Tertiary alcohol.Tertiary alcohol
Primary alcohol.Secondary alcohol.Secondary alcohol.Secondary amine
c1ccc2c(c1)CCC2
C1CCNCC1
C1CCNCC1
HO-
null
null
72
CC(C)O.O=C1c2ccccc2C(=O)C1(O)O.[NH4+]>>OC[C@H]1CNC[C@@H](O)[C@@H]1O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-072ab9e7dac74a0bbec4b4073a868935
OC[C@H]1CNC[C@@H](O)[C@@H]1O>>OC[C@H]1CNC[C@@H](O)[C@@H]1O
C1[C@@H]([C@H]([C@@H](CN1)O)O)CO.Cl>>C1[C@@H]([C@H]([C@@H](CN1)O)O)CO.Cl
[OH:2][CH2:3][C@H:4]1[CH2:5][NH:6][CH2:7][C@@H:8]([OH:9])[C@@H:10]1[OH:11]>>[OH:2][CH2:3][C@H:4]1[CH2:5][NH:6][CH2:7][C@@H:8]([OH:9])[C@@H:10]1[OH:11]
OC[C@H]1CNC[C@@H](O)[C@@H]1O
OC[C@H]1CNC[C@@H](O)[C@@H]1O
null
null
CO.CC(=O)C.C(C)(C)O
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
C1CCNCC1
null
null
[]
null
null
8
HOUR
Isofagomine free base (30 mg) was dissolved in MeOH (5 mL) and 4 N HCl (0.5 mL) in isopropanol and acetone (4.0 mL). The sample was stored refrigerated overnight and filtered. Crystals were observed in the solution. However, when filtered, the product was a yellow substance having a glue-like consistency. Conditions: S...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
C1CCNCC1
null
CO.CC(=O)C.C(C)(C)O
null
8
OC[C@H]1CNC[C@@H](O)[C@@H]1O>CO.CC(=O)C.C(C)(C)O>OC[C@H]1CNC[C@@H](O)[C@@H]1O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-30f01609220f49bf9ce6795f15a73cfa
O=C[C@@H](O)[C@H](O)[C@H](O)CO.OCc1ccccc1>>O=C[C@](O)(Cc1ccccc1)[C@H](O)[C@H](O)CO
O=C[C@@H](O)[C@H](O)[C@H](O)CO.C(C1=CC=CC=C1)O.C(C)(=O)Cl>>C(C1=CC=CC=C1)[C@](C=O)(O)[C@H](O)[C@H](O)CO
[O:1]=[CH:2][C@@H:3]([OH:4])[C@H:12]([OH:13])[C@H:14]([OH:15])[CH2:16][OH:17].O[CH2:5][c:6]1[cH:7][cH:8][cH:9][cH:10][cH:11]1>>[O:1]=[CH:2][C@:3]([OH:4])([CH2:5][c:6]1[cH:7][cH:8][cH:9][cH:10][cH:11]1)[C@H:12]([OH:13])[C@H:14]([OH:15])[CH2:16][OH:17]
O=C[C@@H](O)[C@H](O)[C@H](O)CO.OCc1ccccc1
O=C[C@](O)(Cc1ccccc1)[C@H](O)[C@H](O)CO
null
null
CC(C)(C)OC
C-C Coupling
OtherReaction
f42956668c59a62a2fe14af6f60169215fa9f76b367e8cc8580fced345e044dd
ad507317811a44d17061f0a40d99a489d6f22dc298e6a9d74de85776c8c90e8d
c1ccccc1
O-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[C:5]-[C:6](-[O;D1;H1:7])-[C@H;D3;+0:8](-[O;D1;H1:9])-[C:10]=[O;D1;H0:11]>>[C:5]-[C:6](-[O;D1;H1:7])-[C@;H0;D4;+0:8](-[O;D1;H1:9])(-[C:10]=[O;D1;H0:11])-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
35
CELSIUS
8
HOUR
D-Arabinose (50 kg, 330.04 moles) and benzyl alcohol (132.2 kg, 4.33 equivalents) were stirred and heated to 35° C. Acetyl chloride (10.9 kg, 0.42 equivalents), keeping the temperature <45° C., then stirred 50° C. overnight. The mixture was cooled to 20° C. and diluted with MTBE (600 kg). The mixture was stirred for 0....
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary alcohol
Aldehyde.Tertiary alcohol
null
null
c1ccccc1
HO-
CC(C)(C)OC
35
8
O=C[C@@H](O)[C@H](O)[C@H](O)CO.OCc1ccccc1>CC(C)(C)OC>O=C[C@](O)(Cc1ccccc1)[C@H](O)[C@H](O)CO
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-514b8a8d2cd3433a8ba8ddfb06d0d84a
O=C(O)[C@H](O)[C@@H](O)C(=O)O>>O=C([O-])[C@H](O)[C@@H](O)C(=O)[O-]
C([C@H](O)[C@@H](O)C(=O)O)(=O)O.C1[C@@H]([C@H]([C@@H](CN1)O)O)CO>>C1[C@@H]([C@H]([C@@H](CN1)O)O)CO.C(=O)([O-])[C@H](O)[C@@H](O)C(=O)[O-]
[O:1]=[C:2]([OH:3])[C@H:4]([OH:5])[C@@H:6]([OH:7])[C:8](=[O:9])[OH:10]>>[O:1]=[C:2]([O-:3])[C@H:4]([OH:5])[C@@H:6]([OH:7])[C:8](=[O:9])[O-:10]
O=C(O)[C@H](O)[C@@H](O)C(=O)O
O=C([O-])[C@H](O)[C@@H](O)C(=O)[O-]
null
null
O
Oxidation
OtherReaction
4af04878ecd22d61c6d7d46db52e672904d5e72408231940a5cea872324a16a2
4e878a1fdc9370141a3ed00507bdfaa037f36d163bb15c5076375a9835c80b8f
null
[O;D1;H0:1]=[C:2](-[OH;D1;+0:3])-[C:4]-[C:5]-[C:6](=[O;D1;H0:7])-[OH;D1;+0:8]>>[O-;H0;D1:8]-[C:6](=[O;D1;H0:7])-[C:5]-[C:4]-[C:2](-[O-;H0;D1:3])=[O;D1;H0:1]
137.5
[{"value": 91.0, "product": "C1[C@@H]([C@H]([C@@H](CN1)O)O)CO.C(=O)([O-])[C@H](O)[C@@H](O)C(=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 137.5, "product": "C1[C@@H]([C@H]([C@@H](CN1)O)O)CO.C(=O)([O-])[C@H](O)[C@@H](O)C(=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
10
MINUTE
A solution of L-(+)-tartaric acid (102 mg, 0.679 mmol) in deionized water (1.0 mL) was added into the solution of isofagomine (200 mg, 2.0 equivalents) dissolved in deionized water (2.0 mL) at room temperature. The solution was stirred for 10 min and lyophilized overnight. The residue was further dried under vacuum at ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Carboxylic acid
null
null
null
null
null
O
null
0.166667
O=C(O)[C@H](O)[C@@H](O)C(=O)O>O>O=C([O-])[C@H](O)[C@@H](O)C(=O)[O-]
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-67b86b27891f4c62aced766825510af3
O=C(O)[C@@H](O)[C@H](O)C(=O)O>>O=C([O-])[C@@H](O)[C@H](O)C(=O)[O-]
C([C@@H](O)[C@H](O)C(=O)O)(=O)O.C1[C@@H]([C@H]([C@@H](CN1)O)O)CO>>C1[C@@H]([C@H]([C@@H](CN1)O)O)CO.C(=O)([O-])[C@@H](O)[C@H](O)C(=O)[O-]
[O:1]=[C:2]([OH:3])[C@@H:4]([OH:5])[C@H:6]([OH:7])[C:8](=[O:9])[OH:10]>>[O:1]=[C:2]([O-:3])[C@@H:4]([OH:5])[C@H:6]([OH:7])[C:8](=[O:9])[O-:10]
O=C(O)[C@@H](O)[C@H](O)C(=O)O
O=C([O-])[C@@H](O)[C@H](O)C(=O)[O-]
null
null
O
Oxidation
OtherReaction
4af04878ecd22d61c6d7d46db52e672904d5e72408231940a5cea872324a16a2
4e878a1fdc9370141a3ed00507bdfaa037f36d163bb15c5076375a9835c80b8f
null
[O;D1;H0:1]=[C:2](-[OH;D1;+0:3])-[C:4]-[C:5]-[C:6](=[O;D1;H0:7])-[OH;D1;+0:8]>>[O-;H0;D1:8]-[C:6](=[O;D1;H0:7])-[C:5]-[C:4]-[C:2](-[O-;H0;D1:3])=[O;D1;H0:1]
143.3
[{"value": 95.0, "product": "C1[C@@H]([C@H]([C@@H](CN1)O)O)CO.C(=O)([O-])[C@@H](O)[C@H](O)C(=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 143.3, "product": "C1[C@@H]([C@H]([C@@H](CN1)O)O)CO.C(=O)([O-])[C@@H](O)[C@H](O)C(=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
10
MINUTE
A solution of D-(-)-tartaric acid (102 mg, 0.679 mmol) in deionized water (1.0 mL) was added into the solution of isofagomine (200 mg, 2.0 equivalents) dissolved in deionized water (2.0 mL) at room temperature. The solution was stirred for 10 min and lyophilized overnight. The residue was further dried under vacuum at ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Carboxylic acid
null
null
null
null
null
O
null
0.166667
O=C(O)[C@@H](O)[C@H](O)C(=O)O>O>O=C([O-])[C@@H](O)[C@H](O)C(=O)[O-]