dataset_id
large_stringclasses
414 values
reaction_id
large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
reactant_smiles
large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6adc145dc9574a5abe15a17244a23aab
CCC(=O)C1CCOC1.Nc1ccc([N+](=O)[O-])cn1>>Cc1c(C2CCOC2)nc2ccc([N+](=O)[O-])cn12
O1CC(CC1)C(CC)=O.NC1=NC=C(C=C1)[N+](=O)[O-]>>CC1=C(N=C2N1C=C(C=C2)[N+](=O)[O-])C2COCC2
O=[C:3]([CH2:2][CH3:1])[CH:4]1[CH2:5][CH2:6][O:7][CH2:8]1.[NH2:9][c:10]1[cH:11][cH:12][c:13]([N+:14](=[O:15])[O-:16])[cH:17][n:18]1>>[CH3:1][c:2]1[c:3]([CH:4]2[CH2:5][CH2:6][O:7][CH2:8]2)[n:9][c:10]2[cH:11][cH:12][c:13]([N+:14](=[O:15])[O-:16])[cH:17][n:18]12
CCC(=O)C1CCOC1.Nc1ccc([N+](=O)[O-])cn1
Cc1c(C2CCOC2)nc2ccc([N+](=O)[O-])cn12
null
null
C(C)(=O)OCC
Aromatic Heterocycle Formation
OtherReaction
cbc7e6c5e0a09d2e514fd60fb099adf259bb478395dbd8e339a49821fedd9120
8182c33d66a1c51620dac2e3d5b839c3fec60d5b5668262efc6be8b10c115a58
c1ccn2cc(C3CCOC3)nc2c1
O=[C;H0;D3;+0:1](-[CH2;D2;+0:2]-[C;D1;H3:3])-[C:4](-[C:5])-[C:6]-[#8:7].[NH2;D1;+0:8]-[c:9](:[c:10]):[n;H0;D2;+0:11]:[c:12]:[c:13]>>[#8:7]-[C:6]-[C:4](-[c;H0;D3;+0:1]1:[n;H0;D2;+0:8]:[c:9](:[c:10]):[n;H0;D3;+0:11](:[c:12]:[c:13]):[c;H0;D3;+0:2]:1-[C;D1;H3:3])-[C:5]
null
[]
null
null
null
null
Operations similar to Production Example 1-(1) were conducted using 1-tetrahydro-3-furanyl-1-propanone in place of 3-methyl-2-butanone, and successively those of Production Example 1-(2) were conducted using 2-amino-5-nitropyridine. The resulting solid was suspended in ethyl acetate, washed with saturated aqueous sodiu...
10.6084/m9.figshare.5104873.v1
null
Ketone.Primary amine
null
c1ccncc1
c1ccn2ccnc2c1
C1CCOC1.c1ccn2ccnc2c1
HO-
C(C)(=O)OCC
null
null
CCC(=O)C1CCOC1.Nc1ccc([N+](=O)[O-])cn1>C(C)(=O)OCC>Cc1c(C2CCOC2)nc2ccc([N+](=O)[O-])cn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6c35de7734a0408eaf9404625f6f2ad4
Nc1ccc([N+](=O)[O-])cn1.O=C1CCCCC1Cl>>O=[N+]([O-])c1ccc2nc3c(n2c1)CCCC3
ClC1C(CCCC1)=O.NC1=NC=C(C=C1)[N+](=O)[O-]>>[N+](=O)([O-])C=1C=CC2=NC3=C(N2C1)CCCC3
[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]([NH2:8])[n:11][cH:12]1.O=[C:9]1[CH:10](Cl)[CH2:13][CH2:14][CH2:15][CH2:16]1>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]2[n:8][c:9]3[c:10]([n:11]2[cH:12]1)[CH2:13][CH2:14][CH2:15][CH2:16]3
Nc1ccc([N+](=O)[O-])cn1.O=C1CCCCC1Cl
O=[N+]([O-])c1ccc2nc3c(n2c1)CCCC3
null
null
C(C)(=O)OCC
Aromatic Heterocycle Formation
OtherReaction
7b133ee0fb2f2591e32fd58418cd7b700f192a61eeb5c67e6d9e3075dc440d37
235fd48cd394ba1137abde2ba7484c051be6ffcae187060d6065fe5adf0e90a3
c1ccn2c3c(nc2c1)CCCC3
Cl-[CH;D3;+0:1]1-[C:2]-[C:3]-[C:4]-[C:5]-[C;H0;D3;+0:6]-1=O.[NH2;D1;+0:7]-[c:8](:[c:9]):[n;H0;D2;+0:10]:[c:11]:[c:12]>>[c:12]:[c:11]:[n;H0;D3;+0:10]1:[c:8](:[c:9]):[n;H0;D2;+0:7]:[c;H0;D3;+0:6]2:[c;H0;D3;+0:1]:1-[C:2]-[C:3]-[C:4]-[C:5]-2
null
[]
null
null
null
null
Operations similar to Production Example 1-(2) were conducted using 2-chlorocyclohexanone and 2-amino-5-nitropyridine. The resulting solid was suspended in ethyl acetate, washed with saturated aqueous sodium hydrogencarbonate solution and purified by silica gel column chromatography (hexane/ethyl acetate=2/1) to provid...
10.6084/m9.figshare.5104873.v1
null
Secondary halide.Ketone.Primary amine
null
c1ccncc1.C1CCCCC1
c1ccn2c3c(nc2c1)CCCC3
c1ccn2c3c(nc2c1)CCCC3
HCl
C(C)(=O)OCC
null
null
Nc1ccc([N+](=O)[O-])cn1.O=C1CCCCC1Cl>C(C)(=O)OCC>O=[N+]([O-])c1ccc2nc3c(n2c1)CCCC3
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e5ba5118e66d4f648c4af2bcf4b47e4c
Cc1ccc(S(=O)(=O)Cl)cc1.Nc1ccc([N+](=O)[O-])cn1>>Cc1ccc(S(=O)(=O)Nc2ccc([N+](=O)[O-])cn2)cc1
N1=CC=CC=C1.NC1=NC=C(C=C1)[N+](=O)[O-].C1(=CC=C(C=C1)S(=O)(=O)Cl)C>>CC1=CC=C(C=C1)S(=O)(=O)NC1=NC=C(C=C1)[N+](=O)[O-]
Cl[S:6]([c:5]1[cH:4][cH:3][c:2]([CH3:1])[cH:20][cH:19]1)(=[O:7])=[O:8].[NH2:9][c:10]1[cH:11][cH:12][c:13]([N+:14](=[O:15])[O-:16])[cH:17][n:18]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([S:6](=[O:7])(=[O:8])[NH:9][c:10]2[cH:11][cH:12][c:13]([N+:14](=[O:15])[O-:16])[cH:17][n:18]2)[cH:19][cH:20]1
Cc1ccc(S(=O)(=O)Cl)cc1.Nc1ccc([N+](=O)[O-])cn1
Cc1ccc(S(=O)(=O)Nc2ccc([N+](=O)[O-])cn2)cc1
null
null
O
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
84f0a2c480e4021adb28613388cdf35ca03a8bd65bbdad356e160a1b94684976
2988afdf4a13d931f021994343ac8648c6e63ca3a4c0ba598a4b99bbffc001c8
O=S(=O)(Nc1ccccn1)c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[NH2;D1;+0:7]-[c:8](:[c:9]):[#7;a:10]:[c:11]>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[NH;D2;+0:7]-[c:8](:[c:9]):[#7;a:10]:[c:11])-[c:4](:[c:5]):[c:6]
79.4
[{"value": 79.4, "product": "CC1=CC=C(C=C1)S(=O)(=O)NC1=NC=C(C=C1)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
null
null
A pyridine suspension (40 ml) containing 2-amino-5-nitropyridine (4.0 g) and p-toluenesulfonyl chloride (5.7 g) was stirred for a day and night at 100° C. The reaction liquid was poured in water (200 ml), the precipitated solid was recovered by filtration, and successively washed with water and diethyl ether by the ord...
10.6084/m9.figshare.5104873.v1
null
Tosylate.Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccccc1.c1ccncc1
HCl
O
100
null
Cc1ccc(S(=O)(=O)Cl)cc1.Nc1ccc([N+](=O)[O-])cn1>O>Cc1ccc(S(=O)(=O)Nc2ccc([N+](=O)[O-])cn2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d8faafe0a96540189e61256568c08fed
FC(F)(F)c1ccc(Br)cc1.O=C(O)c1ccc(B(O)O)cc1>>O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1
BrC1=CC=C(C=C1)C(F)(F)F.C(=O)(O)C1=CC=C(C=C1)B(O)O>>FC(C1=CC=C(C=C1)C1=CC=C(C=C1)C(=O)O)(F)F
Br[c:8]1[cH:9][cH:10][c:11]([C:12]([F:13])([F:14])[F:15])[cH:16][cH:17]1.OB(O)[c:7]1[cH:6][cH:5][c:4]([C:2](=[O:1])[OH:3])[cH:19][cH:18]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][c:11]([C:12]([F:13])([F:14])[F:15])[cH:16][cH:17]2)[cH:18][cH:19]1
FC(F)(F)c1ccc(Br)cc1.O=C(O)c1ccc(B(O)O)cc1
O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
COCCOC
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccccc2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:5]:[c:4]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:2]:[c:3]
71
[{"value": 71.0, "product": "FC(C1=CC=C(C=C1)C1=CC=C(C=C1)C(=O)O)(F)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
null
null
To a mixed solution of ethylene glycol dimethyl ether (400 ml)-2M aqueous sodium carbonate solution (80 ml), 4-bromobenzotrifluoride (5.0 g), 4-carboxyphenylboronic acid (3.9 g) and tetrakistriphenylphosphinepalladium (2.5 g) were added and stirred at 100° C. for a day and night. Concentrating the reaction liquid under...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.COCCOC
100
null
FC(F)(F)c1ccc(Br)cc1.O=C(O)c1ccc(B(O)O)cc1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.COCCOC>O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-75fa72349d064702bc2f10d81a0d521d
Cc1cc(C(=O)O)ccc1Br.OB(O)c1ccc(C(F)(F)F)cc1>>Cc1cc(C(=O)O)ccc1-c1ccc(C(F)(F)F)cc1
FC(C1=CC=C(C=C1)B(O)O)(F)F.BrC1=C(C=C(C=C1)C(=O)O)C>>CC1=C(C=CC(=C1)C(=O)O)C1=CC=C(C=C1)C(F)(F)F
Br[c:10]1[c:2]([CH3:1])[cH:3][c:4]([C:5](=[O:6])[OH:7])[cH:8][cH:9]1.OB(O)[c:11]1[cH:12][cH:13][c:14]([C:15]([F:16])([F:17])[F:18])[cH:19][cH:20]1>>[CH3:1][c:2]1[cH:3][c:4]([C:5](=[O:6])[OH:7])[cH:8][cH:9][c:10]1-[c:11]1[cH:12][cH:13][c:14]([C:15]([F:16])([F:17])[F:18])[cH:19][cH:20]1
Cc1cc(C(=O)O)ccc1Br.OB(O)c1ccc(C(F)(F)F)cc1
Cc1cc(C(=O)O)ccc1-c1ccc(C(F)(F)F)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccccc2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[C;D1;H3:5]):[c:6].O-B(-O)-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10]:[c:11]>>[C;D1;H3:5]-[c:4](:[c:6]):[c;H0;D3;+0:1](-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10]:[c:11]):[c:2]:[c:3]
null
[]
null
null
null
null
Production Example 14 was repeated except that 4-(trifluoromethyl)phenylboronic acid and 4-bromo-3-methylbenzenecarboxylic acid were used, to provide the title compound as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
HBr.B
null
null
null
Cc1cc(C(=O)O)ccc1Br.OB(O)c1ccc(C(F)(F)F)cc1>>Cc1cc(C(=O)O)ccc1-c1ccc(C(F)(F)F)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c01d2bd09a234c93973e07e594693927
O=C(O)c1ccc(Br)cc1F.OB(O)c1ccc(C(F)(F)F)cc1>>O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1F
FC(C1=CC=C(C=C1)B(O)O)(F)F.BrC1=CC(=C(C=C1)C(=O)O)F>>FC=1C=C(C=CC1C(=O)O)C1=CC=C(C=C1)C(F)(F)F
Br[c:7]1[cH:6][cH:5][c:4]([C:2](=[O:1])[OH:3])[c:19]([F:20])[cH:18]1.OB(O)[c:8]1[cH:9][cH:10][c:11]([C:12]([F:13])([F:14])[F:15])[cH:16][cH:17]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][c:11]([C:12]([F:13])([F:14])[F:15])[cH:16][cH:17]2)[cH:18][c:19]1[F:20]
O=C(O)c1ccc(Br)cc1F.OB(O)c1ccc(C(F)(F)F)cc1
O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1F
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccccc2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:10]:[c:9]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:7]:[c:8]
null
[]
null
null
null
null
Production Example 14 was repeated except that 4-(trifluoromethyl)phenylboronic acid and 4-bromo-2-fluorobenzenecarboxylic acid were used, to provide the title compound as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
HBr.B
null
null
null
O=C(O)c1ccc(Br)cc1F.OB(O)c1ccc(C(F)(F)F)cc1>>O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1F
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-273cf6a0dc324d5bb169ee6b263492f1
Brc1ccccn1.O=C(O)c1ccc(B(O)O)cc1>>O=C(O)c1ccc(-c2ccccn2)cc1
C(=O)(O)C1=CC=C(C=C1)B(O)O.BrC1=NC=CC=C1>>N1=C(C=CC=C1)C1=CC=C(C=C1)C(=O)O
Br[c:8]1[cH:9][cH:10][cH:11][cH:12][n:13]1.OB(O)[c:7]1[cH:6][cH:5][c:4]([C:2](=[O:1])[OH:3])[cH:15][cH:14]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][cH:11][cH:12][n:13]2)[cH:14][cH:15]1
Brc1ccccn1.O=C(O)c1ccc(B(O)O)cc1
O=C(O)c1ccc(-c2ccccn2)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
07e9b6e71d806aa92d4573f3838e77c7c8344de3e5d5735ebdb5fc6862ebf27d
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccccn2)cc1
Br-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:5]:[c:4]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[#7;a:2]:[c:3]
null
[]
null
null
null
null
Production Example 14 was repeated except that 4-carboxyphenylboronic acid and 2-bromopyridine were used, to provide the title compound as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccncc1.c1ccccc1
c1ccccc1.c1ccncc1
c1ccccc1.c1ccncc1
HBr.B
null
null
null
Brc1ccccn1.O=C(O)c1ccc(B(O)O)cc1>>O=C(O)c1ccc(-c2ccccn2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-219a172ed1f541e9964bc63f0fbf5490
COC(=O)c1ccc(B(O)O)cc1.Cc1ccc(Br)nc1>>COC(=O)c1ccc(-c2ccc(C)cn2)cc1
COC(=O)C1=CC=C(C=C1)B(O)O.BrC1=NC=C(C=C1)C>>CC=1C=CC(=NC1)C1=CC=C(C(=O)OC)C=C1
OB(O)[c:8]1[cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:17][cH:16]1.Br[c:9]1[cH:10][cH:11][c:12]([CH3:13])[cH:14][n:15]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8](-[c:9]2[cH:10][cH:11][c:12]([CH3:13])[cH:14][n:15]2)[cH:16][cH:17]1
COC(=O)c1ccc(B(O)O)cc1.Cc1ccc(Br)nc1
COC(=O)c1ccc(-c2ccc(C)cn2)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
07e9b6e71d806aa92d4573f3838e77c7c8344de3e5d5735ebdb5fc6862ebf27d
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccccn2)cc1
Br-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:5]:[c:4]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[#7;a:2]:[c:3]
null
[]
null
null
null
null
Repeating the operations of Production Example 14 using 4-(methoxycarbonyl)phenylboronic acid and 2-bromo-5-methylpyridine, methyl 4-(5-methyl-2-pyridyl)benzoate was obtained. Hydrolyzing the same with 5N aqueous sodium hydroxide solution, the title compound was obtained as white solid. Conditions: See reaction.notes.p...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccncc1
c1ccccc1.c1ccncc1
c1ccccc1.c1ccncc1
HBr.B
null
null
null
COC(=O)c1ccc(B(O)O)cc1.Cc1ccc(Br)nc1>>COC(=O)c1ccc(-c2ccc(C)cn2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-aa062152557a40419e3d9d16e682ccd0
COC(=O)c1ccc(B(O)O)cc1.Clc1ccc(Cl)nc1>>COC(=O)c1ccc(-c2ccc(Cl)cn2)cc1
COC(=O)C1=CC=C(C=C1)B(O)O.ClC1=NC=C(C=C1)Cl>>ClC=1C=CC(=NC1)C1=CC=C(C(=O)OC)C=C1
OB(O)[c:8]1[cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:17][cH:16]1.Cl[c:9]1[cH:10][cH:11][c:12]([Cl:13])[cH:14][n:15]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8](-[c:9]2[cH:10][cH:11][c:12]([Cl:13])[cH:14][n:15]2)[cH:16][cH:17]1
COC(=O)c1ccc(B(O)O)cc1.Clc1ccc(Cl)nc1
COC(=O)c1ccc(-c2ccc(Cl)cn2)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
07e9b6e71d806aa92d4573f3838e77c7c8344de3e5d5735ebdb5fc6862ebf27d
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccccn2)cc1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:5]:[c:4]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[#7;a:2]:[c:3]
null
[]
null
null
null
null
Repeating the operations of Production Example 14 using 4-(methoxycarbonyl)phenylboronic acid and 2,5-dichloropyridine, methyl 4-(5-chloro-2-pyridyl)benzoate was obtained. Hydrolyzing the same with 5N aqueous sodium hydroxide solution, the title compound was obtained as white solid. Conditions: See reaction.notes.proce...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccncc1
c1ccccc1.c1ccncc1
c1ccccc1.c1ccncc1
HCl.B
null
null
null
COC(=O)c1ccc(B(O)O)cc1.Clc1ccc(Cl)nc1>>COC(=O)c1ccc(-c2ccc(Cl)cn2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b6e20f7995304c27b8b041e69c372c87
COC(=O)c1ccc(B(O)O)cc1.COc1ccc(Br)nc1>>COC(=O)c1ccc(-c2ccc(OC)cn2)cc1
COC(=O)C1=CC=C(C=C1)B(O)O.BrC1=NC=C(C=C1)OC>>COC=1C=CC(=NC1)C1=CC=C(C(=O)OC)C=C1
OB(O)[c:8]1[cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:18][cH:17]1.Br[c:9]1[cH:10][cH:11][c:12]([O:13][CH3:14])[cH:15][n:16]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8](-[c:9]2[cH:10][cH:11][c:12]([O:13][CH3:14])[cH:15][n:16]2)[cH:17][cH:18]1
COC(=O)c1ccc(B(O)O)cc1.COc1ccc(Br)nc1
COC(=O)c1ccc(-c2ccc(OC)cn2)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
07e9b6e71d806aa92d4573f3838e77c7c8344de3e5d5735ebdb5fc6862ebf27d
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccccn2)cc1
Br-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:5]:[c:4]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[#7;a:2]:[c:3]
null
[]
null
null
null
null
Repeating the operations of Production Example 14 using 4-(methoxycarbonyl)phenylboronic acid and 2-bromo-5-methoxypyridine, methyl 4-(5-methoxy-2-pyridyl)benzoate was obtained. Hydrolyzing the same with 5N aqueous sodium hydroxide solution, the title compound was obtained as white solid. Conditions: See reaction.notes...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccncc1
c1ccccc1.c1ccncc1
c1ccccc1.c1ccncc1
HBr.B
null
null
null
COC(=O)c1ccc(B(O)O)cc1.COc1ccc(Br)nc1>>COC(=O)c1ccc(-c2ccc(OC)cn2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-813bc511fa8c488fbc2de6d165096ca0
FC(F)c1ccc(Br)cn1.O=C(O)c1ccc(B(O)O)cc1>>O=C(O)c1ccc(-c2ccc(C(F)F)nc2)cc1
C(=O)(O)C1=CC=C(C=C1)B(O)O.BrC=1C=CC(=NC1)C(F)F>>FC(C1=CC=C(C=N1)C1=CC=C(C=C1)C(=O)O)F
Br[c:8]1[cH:9][cH:10][c:11]([CH:12]([F:13])[F:14])[n:15][cH:16]1.OB(O)[c:7]1[cH:6][cH:5][c:4]([C:2](=[O:1])[OH:3])[cH:18][cH:17]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][c:11]([CH:12]([F:13])[F:14])[n:15][cH:16]2)[cH:17][cH:18]1
FC(F)c1ccc(Br)cn1.O=C(O)c1ccc(B(O)O)cc1
O=C(O)c1ccc(-c2ccc(C(F)F)nc2)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
07e9b6e71d806aa92d4573f3838e77c7c8344de3e5d5735ebdb5fc6862ebf27d
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2cccnc2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]:[c:6]:1.O-B(-O)-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10]:[c:11]>>[c:9]:[c:8]:[c;H0;D3;+0:7](-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]:[c:6]:1):[c:10]:[c:11]
null
[]
null
null
null
null
Operations similar to those of Production Example 14 were conducted using 4-carboxyphenylboronic acid and 5-bromo-2-(difluoromethyl)pyridine, to provide the title compound as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccncc1.c1ccccc1
c1ccccc1.c1ccncc1
c1ccccc1.c1ccncc1
HBr.B
null
null
null
FC(F)c1ccc(Br)cn1.O=C(O)c1ccc(B(O)O)cc1>>O=C(O)c1ccc(-c2ccc(C(F)F)nc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b62752ee596f4f8c86b7587014a8b2bd
FC(F)Oc1ccc(Br)nc1.O=C(O)c1ccc(B(O)O)cc1>>O=C(O)c1ccc(-c2ccc(OC(F)F)cn2)cc1
C(=O)(O)C1=CC=C(C=C1)B(O)O.BrC1=NC=C(C=C1)OC(F)F>>FC(OC=1C=CC(=NC1)C1=CC=C(C=C1)C(=O)O)F
Br[c:8]1[cH:9][cH:10][c:11]([O:12][CH:13]([F:14])[F:15])[cH:16][n:17]1.OB(O)[c:7]1[cH:6][cH:5][c:4]([C:2](=[O:1])[OH:3])[cH:19][cH:18]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][c:11]([O:12][CH:13]([F:14])[F:15])[cH:16][n:17]2)[cH:18][cH:19]1
FC(F)Oc1ccc(Br)nc1.O=C(O)c1ccc(B(O)O)cc1
O=C(O)c1ccc(-c2ccc(OC(F)F)cn2)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
07e9b6e71d806aa92d4573f3838e77c7c8344de3e5d5735ebdb5fc6862ebf27d
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccccn2)cc1
Br-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:5]:[c:4]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[#7;a:2]:[c:3]
null
[]
null
null
null
null
Operations similar to those of Production Example 14 were conducted using 4-carboxyphenylboronic acid and 2-bromo-5-(difluoromethoxy)pyridine, to provide the title compound as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccncc1.c1ccccc1
c1ccccc1.c1ccncc1
c1ccccc1.c1ccncc1
HBr.B
null
null
null
FC(F)Oc1ccc(Br)nc1.O=C(O)c1ccc(B(O)O)cc1>>O=C(O)c1ccc(-c2ccc(OC(F)F)cn2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d32d41c62af2483c8f0d709efb1581f4
O=C(O)c1ccc(Cl)nc1.OB(O)c1ccc(F)cc1>>O=C(O)c1ccc(-c2ccc(F)cc2)nc1
ClC1=NC=C(C(=O)O)C=C1.FC1=CC=C(C=C1)B(O)O>>FC1=CC=C(C=C1)C1=NC=C(C(=O)O)C=C1
Cl[c:7]1[cH:6][cH:5][c:4]([C:2](=[O:1])[OH:3])[cH:16][n:15]1.OB(O)[c:8]1[cH:9][cH:10][c:11]([F:12])[cH:13][cH:14]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][c:11]([F:12])[cH:13][cH:14]2)[n:15][cH:16]1
O=C(O)c1ccc(Cl)nc1.OB(O)c1ccc(F)cc1
O=C(O)c1ccc(-c2ccc(F)cc2)nc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
07e9b6e71d806aa92d4573f3838e77c7c8344de3e5d5735ebdb5fc6862ebf27d
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccccn2)cc1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:10]:[c:9]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5]):[c:7]:[c:8]
null
[]
null
null
null
null
Operations similar to those of Production Example 14 were conducted using 6-chloronicotinic acid and 4-fluorophenylboronic acid, to provide the title compound as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccncc1.c1ccccc1
c1ccncc1.c1ccccc1
c1ccncc1.c1ccccc1
HCl.B
null
null
null
O=C(O)c1ccc(Cl)nc1.OB(O)c1ccc(F)cc1>>O=C(O)c1ccc(-c2ccc(F)cc2)nc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-cb7c899b325548aa861fe8f1f8dc9983
O=C(O)c1ccc(Br)cn1.OB(O)c1ccc(F)cc1>>O=C(O)c1ccc(-c2ccc(F)cc2)cn1
BrC=1C=CC(=NC1)C(=O)O.FC1=CC=C(C=C1)B(O)O>>FC1=CC=C(C=C1)C=1C=CC(=NC1)C(=O)O
Br[c:7]1[cH:6][cH:5][c:4]([C:2](=[O:1])[OH:3])[n:16][cH:15]1.OB(O)[c:8]1[cH:9][cH:10][c:11]([F:12])[cH:13][cH:14]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][c:11]([F:12])[cH:13][cH:14]2)[cH:15][n:16]1
O=C(O)c1ccc(Br)cn1.OB(O)c1ccc(F)cc1
O=C(O)c1ccc(-c2ccc(F)cc2)cn1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
07e9b6e71d806aa92d4573f3838e77c7c8344de3e5d5735ebdb5fc6862ebf27d
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2cccnc2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4](-[C:5](=[O;D1;H0:6])-[O;D1;H1:7]):[c:8]:[c:9]:1.O-B(-O)-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]>>[O;D1;H0:6]=[C:5](-[O;D1;H1:7])-[c:4]1:[#7;a:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]):[c:9]:[c:8]:1
null
[]
null
null
null
null
Operations similar to those of Production Example 14 were conducted using 5-bromo-2-pyridinecarboxylic acid and 4-fluorophenylboronic acid, to provide the title compound as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccncc1.c1ccccc1
c1ccncc1.c1ccccc1
c1ccncc1.c1ccccc1
HBr.B
null
null
null
O=C(O)c1ccc(Br)cn1.OB(O)c1ccc(F)cc1>>O=C(O)c1ccc(-c2ccc(F)cc2)cn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e4c9e6e11d9449da9308875330f71e1e
Nc1cnc(Br)cn1.OB(O)c1ccc(F)cc1>>Nc1cnc(-c2ccc(F)cc2)cn1
NC1=NC=C(N=C1)Br.FC1=CC=C(C=C1)B(O)O>>NC1=NC=C(N=C1)C1=CC=C(C=C1)F
Br[c:5]1[n:4][cH:3][c:2]([NH2:1])[n:14][cH:13]1.OB(O)[c:6]1[cH:7][cH:8][c:9]([F:10])[cH:11][cH:12]1>>[NH2:1][c:2]1[cH:3][n:4][c:5](-[c:6]2[cH:7][cH:8][c:9]([F:10])[cH:11][cH:12]2)[cH:13][n:14]1
Nc1cnc(Br)cn1.OB(O)c1ccc(F)cc1
Nc1cnc(-c2ccc(F)cc2)cn1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
f4f2599a1f2d23f122d9e68430d5dc3c8a9f800f7adcc4136d8b17b1c1c7d091
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2cnccn2)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5]:[c:6]:1.O-B(-O)-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10]:[c:11]>>[c:9]:[c:8]:[c;H0;D3;+0:7](-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5]:[c:6]:1):[c:10]:[c:11]
null
[]
null
null
null
null
Conducting the operations similar to those of Production Example 14 using 2-amino-5-bromopyrazine (2.7 g) and 4-fluorophenylboronic acid (3.4 g), 2-amino-5-(4-fluorophenyl)pyrazine was obtained as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1cnccn1.c1ccccc1
c1cnccn1.c1ccccc1
c1cnccn1.c1ccccc1
HBr.B
null
null
null
Nc1cnc(Br)cn1.OB(O)c1ccc(F)cc1>>Nc1cnc(-c2ccc(F)cc2)cn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c5a303d6deb74c0b93190cb64720a986
O=C(O)c1ncc(Br)cn1.OB(O)c1ccccc1>>O=C(O)c1ncc(-c2ccccc2)cn1
BrC=1C=NC(=NC1)C(=O)O.C1(=CC=CC=C1)B(O)O>>C1(=CC=CC=C1)C=1C=NC(=NC1)C(=O)O
Br[c:7]1[cH:6][n:5][c:4]([C:2](=[O:1])[OH:3])[n:15][cH:14]1.OB(O)[c:8]1[cH:9][cH:10][cH:11][cH:12][cH:13]1>>[O:1]=[C:2]([OH:3])[c:4]1[n:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][cH:11][cH:12][cH:13]2)[cH:14][n:15]1
O=C(O)c1ncc(Br)cn1.OB(O)c1ccccc1
O=C(O)c1ncc(-c2ccccc2)cn1
null
null
null
C-C Coupling
Suzuki
5efc69cb0f56c6c241a71b9df28c03b094ed8fc2f31567997f12f88c03083478
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2cncnc2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4](-[C:5](=[O;D1;H0:6])-[O;D1;H1:7]):[#7;a:8]:[c:9]:1.O-B(-O)-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]>>[O;D1;H0:6]=[C:5](-[O;D1;H1:7])-[c:4]1:[#7;a:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]):[c:9]:[#7;a:8]:1
null
[]
null
null
null
null
Conducting the operations similar to those of Production Example 14 using 5-bromopyrimidine-2-carboxylic acid and phenylboronic acid, the title compound was obtained as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1cncnc1.c1ccccc1
c1cncnc1.c1ccccc1
c1cncnc1.c1ccccc1
HBr.B
null
null
null
O=C(O)c1ncc(Br)cn1.OB(O)c1ccccc1>>O=C(O)c1ncc(-c2ccccc2)cn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b274ef78305f4bec9deccbe1812eac39
O=C(O)c1ncc(Br)cn1.OB(O)c1ccc(F)cc1>>O=C(O)c1ncc(-c2ccc(F)cc2)cn1
BrC=1C=NC(=NC1)C(=O)O.FC1=CC=C(C=C1)B(O)O>>FC1=CC=C(C=C1)C=1C=NC(=NC1)C(=O)O
Br[c:7]1[cH:6][n:5][c:4]([C:2](=[O:1])[OH:3])[n:16][cH:15]1.OB(O)[c:8]1[cH:9][cH:10][c:11]([F:12])[cH:13][cH:14]1>>[O:1]=[C:2]([OH:3])[c:4]1[n:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][c:11]([F:12])[cH:13][cH:14]2)[cH:15][n:16]1
O=C(O)c1ncc(Br)cn1.OB(O)c1ccc(F)cc1
O=C(O)c1ncc(-c2ccc(F)cc2)cn1
null
null
null
C-C Coupling
Suzuki
5efc69cb0f56c6c241a71b9df28c03b094ed8fc2f31567997f12f88c03083478
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2cncnc2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4](-[C:5](=[O;D1;H0:6])-[O;D1;H1:7]):[#7;a:8]:[c:9]:1.O-B(-O)-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]>>[O;D1;H0:6]=[C:5](-[O;D1;H1:7])-[c:4]1:[#7;a:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]):[c:9]:[#7;a:8]:1
null
[]
null
null
null
null
Conducting the operations similar to those of Production Example 14 using 5-bromopyrimidine-2-carboxylic acid and 4-fluorophenylboronic acid, the title compound was obtained as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1cncnc1.c1ccccc1
c1cncnc1.c1ccccc1
c1cncnc1.c1ccccc1
HBr.B
null
null
null
O=C(O)c1ncc(Br)cn1.OB(O)c1ccc(F)cc1>>O=C(O)c1ncc(-c2ccc(F)cc2)cn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6f119b61d4c9409ea3a8cfb2e1e3c18d
O=C(O)c1ncc(Br)cn1.OB(O)c1ccc(F)nc1>>O=C(O)c1ncc(-c2ccc(F)nc2)cn1
BrC=1C=NC(=NC1)C(=O)O.FC1=CC=C(C=N1)B(O)O>>FC1=CC=C(C=N1)C=1C=NC(=NC1)C(=O)O
Br[c:7]1[cH:6][n:5][c:4]([C:2](=[O:1])[OH:3])[n:16][cH:15]1.OB(O)[c:8]1[cH:9][cH:10][c:11]([F:12])[n:13][cH:14]1>>[O:1]=[C:2]([OH:3])[c:4]1[n:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][c:11]([F:12])[n:13][cH:14]2)[cH:15][n:16]1
O=C(O)c1ncc(Br)cn1.OB(O)c1ccc(F)nc1
O=C(O)c1ncc(-c2ccc(F)nc2)cn1
null
null
null
C-C Coupling
Suzuki
51855f0568b0c9a2f03c51034f8881daa4aef477007bbafb8803ff38f26b4c50
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1cncc(-c2cncnc2)c1
Br-[c;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4](-[C:5](=[O;D1;H0:6])-[O;D1;H1:7]):[#7;a:8]:[c:9]:1.O-B(-O)-[c;H0;D3;+0:10]1:[c:11]:[#7;a:12]:[c:13]:[c:14]:[c:15]:1>>[O;D1;H0:6]=[C:5](-[O;D1;H1:7])-[c:4]1:[#7;a:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:10]2:[c:11]:[#7;a:12]:[c:13]:[c:14]:[c:15]:2):[c:9]:[#7;a:8]:1
null
[]
null
null
null
null
Conducting the operations similar to those of Production Example 14 using 5-bromopyrimidine-2-carboxylic acid and 6-fluoro-3-pyridineboronic acid, the title compound was obtained as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1cncnc1.c1ccncc1
c1cncnc1.c1ccncc1
c1cncnc1.c1ccncc1
HBr.B
null
null
null
O=C(O)c1ncc(Br)cn1.OB(O)c1ccc(F)nc1>>O=C(O)c1ncc(-c2ccc(F)nc2)cn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-77e5cd59cb334e53be89678974c2cb6b
CC(C)c1cn2cc([N+](=O)[O-])ccc2n1>>CC(C)c1cn2cc(N)ccc2n1
[H][H].Br.C(C)(C)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1>>Br.NC=1C=CC=2N(C1)C=C(N2)C(C)C
O=[N+:10]([O-])[c:9]1[cH:8][n:7]2[cH:6][c:5]([CH:3]([CH3:2])[CH3:4])[n:14][c:13]2[cH:12][cH:11]1>>[CH3:2][CH:3]([CH3:4])[c:5]1[cH:6][n:7]2[cH:8][c:9]([NH2:10])[cH:11][cH:12][c:13]2[n:14]1
CC(C)c1cn2cc([N+](=O)[O-])ccc2n1
CC(C)c1cn2cc(N)ccc2n1
null
[Pd]
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccn2ccnc2c1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]:[#7;a:5]1:[c:6]:[#7;a:7]:[c:8]:[c:9]:1>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]:[#7;a:5]1:[c:6]:[#7;a:7]:[c:8]:[c:9]:1
99.7
[{"value": 99.7, "product": "Br.NC=1C=CC=2N(C1)C=C(N2)C(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a methanol solution (20 ml) containing 2-isopropyl-6-nitroimidazo[1,2-a]pyridine hydrobromide (280 mg), 10% palladium-on-carbon (30 mg) was added, and inside the reaction system was substituted with hydrogen, followed by an hour's stirring at room temperature. The reaction liquid was filtered through Celite™. Concen...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccn2ccnc2c1
Other
[Pd].CO
null
null
CC(C)c1cn2cc([N+](=O)[O-])ccc2n1>[Pd].CO>CC(C)c1cn2cc(N)ccc2n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d377743f8c224d618db6e7cc8d9e42ca
CC(C)c1cn2cc([N+](=O)[O-])ccc2n1.O=C(O)c1ccc(-c2ccc(F)cc2)cc1>>CC(C)c1cn2cc(NC(=O)c3ccc(-c4ccc(F)cc4)cc3)ccc2n1
Br.C(C)(C)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1.FC1=CC=C(C=C1)C1=CC=C(C=C1)C(=O)O>>FC1=CC=C(C=C1)C1=CC=C(C=C1)C(=O)NC=1C=CC=2N(C1)C=C(N2)C(C)C
O=[N+:9]([O-])[c:8]1[cH:7][n:6]2[cH:5][c:4]([CH:2]([CH3:1])[CH3:3])[n:28][c:27]2[cH:26][cH:25]1.O[C:10](=[O:11])[c:12]1[cH:13][cH:14][c:15](-[c:16]2[cH:17][cH:18][c:19]([F:20])[cH:21][cH:22]2)[cH:23][cH:24]1>>[CH3:1][CH:2]([CH3:3])[c:4]1[cH:5][n:6]2[cH:7][c:8]([NH:9][C:10](=[O:11])[c:12]3[cH:13][cH:14][c:15](-[c:16]4[c...
CC(C)c1cn2cc([N+](=O)[O-])ccc2n1.O=C(O)c1ccc(-c2ccc(F)cc2)cc1
CC(C)c1cn2cc(NC(=O)c3ccc(-c4ccc(F)cc4)cc3)ccc2n1
null
null
null
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nccn2c1)c1ccc(-c2ccccc2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[N+;H0;D3:6](-[O-])-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[#7;a:12]:[c:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[#7;a:12]:[c:13]:[c:14]:1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
Conducting the operations similar to those of Example 1 using 2-isopropyl-6-nitroimidazo[1,2-a]pyridine hydrobromide and 4′-fluoro[1,1′-biphenyl]-4-carboxylic acid, the title compound was obtained as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
c1ccn2ccnc2c1.c1ccccc1.c1ccccc1
Other
null
null
null
CC(C)c1cn2cc([N+](=O)[O-])ccc2n1.O=C(O)c1ccc(-c2ccc(F)cc2)cc1>>CC(C)c1cn2cc(NC(=O)c3ccc(-c4ccc(F)cc4)cc3)ccc2n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a69300b5d7a74e068179e9b4bf9f57aa
Cc1nc2ccc([N+](=O)[O-])cn2c1C.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1>>Cc1nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cc4)cc3)cn2c1C
CC=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1C.FC(C1=CC=C(C=C1)C1=CC=C(C=C1)C(=O)O)(F)F>>CC=1N=C2N(C=C(C=C2)NC(=O)C2=CC=C(C=C2)C2=CC=C(C=C2)C(F)(F)F)C1C
O=[N+:8]([O-])[c:7]1[cH:6][cH:5][c:4]2[n:3][c:2]([CH3:1])[c:29]([CH3:30])[n:28]2[cH:27]1.O[C:9](=[O:10])[c:11]1[cH:12][cH:13][c:14](-[c:15]2[cH:16][cH:17][c:18]([C:19]([F:20])([F:21])[F:22])[cH:23][cH:24]2)[cH:25][cH:26]1>>[CH3:1][c:2]1[n:3][c:4]2[cH:5][cH:6][c:7]([NH:8][C:9](=[O:10])[c:11]3[cH:12][cH:13][c:14](-[c:15]...
Cc1nc2ccc([N+](=O)[O-])cn2c1C.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1
Cc1nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cc4)cc3)cn2c1C
null
null
null
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nccn2c1)c1ccc(-c2ccccc2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[N+;H0;D3:6](-[O-])-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
Conducting the operations similar to those of Example 1 using 2,3-dimethyl-6-nitroimidazo[1,2-a]pyridine and 4′-(trifluoromethyl)-[1,1′-biphenyl]-4-carboxylic acid, the title compound was obtained as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
c1ccn2ccnc2c1.c1ccccc1.c1ccccc1
Other
null
null
null
Cc1nc2ccc([N+](=O)[O-])cn2c1C.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1>>Cc1nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cc4)cc3)cn2c1C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-aa58958213264d5881885ba6b7704af5
Cc1cnc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1>>Cc1cnc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cc4)cc3)cn12
CC1=CN=C2N1C=C(C=C2)[N+](=O)[O-].FC(C1=CC=C(C=C1)C1=CC=C(C=C1)C(=O)O)(F)F>>CC1=CN=C2N1C=C(C=C2)NC(=O)C2=CC=C(C=C2)C2=CC=C(C=C2)C(F)(F)F
O=[N+:9]([O-])[c:8]1[cH:7][cH:6][c:5]2[n:4][cH:3][c:2]([CH3:1])[n:29]2[cH:28]1.O[C:10](=[O:11])[c:12]1[cH:13][cH:14][c:15](-[c:16]2[cH:17][cH:18][c:19]([C:20]([F:21])([F:22])[F:23])[cH:24][cH:25]2)[cH:26][cH:27]1>>[CH3:1][c:2]1[cH:3][n:4][c:5]2[cH:6][cH:7][c:8]([NH:9][C:10](=[O:11])[c:12]3[cH:13][cH:14][c:15](-[c:16]4[...
Cc1cnc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1
Cc1cnc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cc4)cc3)cn12
null
null
null
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nccn2c1)c1ccc(-c2ccccc2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[N+;H0;D3:6](-[O-])-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
Conducting the operations similar to those of Example 1 using 3-methyl-6-nitroimidazo[1,2-a]pyridine and 4′-(trifluoromethyl)-[1,1′-biphenyl]-4-carboxylic acid, the title compound was obtained as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
c1ccn2ccnc2c1.c1ccccc1.c1ccccc1
Other
null
null
null
Cc1cnc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1>>Cc1cnc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cc4)cc3)cn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3c23d63b115b4e2c8c297b0fec9a09d8
O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1.O=[N+]([O-])c1ccc2nc3c(n2c1)CCCC3>>O=C(Nc1ccc2nc3c(n2c1)CCCC3)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1
[N+](=O)([O-])C=1C=CC2=NC3=C(N2C1)CCCC3.FC(C1=CC=C(C=C1)C1=CC=C(C=C1)C(=O)O)(F)F>>C1=C(C=CC2=NC3=C(N21)CCCC3)NC(=O)C3=CC=C(C=C3)C3=CC=C(C=C3)C(F)(F)F
O[C:2](=[O:1])[c:17]1[cH:18][cH:19][c:20](-[c:21]2[cH:22][cH:23][c:24]([C:25]([F:26])([F:27])[F:28])[cH:29][cH:30]2)[cH:31][cH:32]1.O=[N+:3]([O-])[c:4]1[cH:5][cH:6][c:7]2[n:8][c:9]3[c:10]([n:11]2[cH:12]1)[CH2:13][CH2:14][CH2:15][CH2:16]3>>[O:1]=[C:2]([NH:3][c:4]1[cH:5][cH:6][c:7]2[n:8][c:9]3[c:10]([n:11]2[cH:12]1)[CH2:...
O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1.O=[N+]([O-])c1ccc2nc3c(n2c1)CCCC3
O=C(Nc1ccc2nc3c(n2c1)CCCC3)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1
null
null
null
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nc3c(n2c1)CCCC3)c1ccc(-c2ccccc2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[N+;H0;D3:6](-[O-])-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
Conducting the operations similar to those of Example 1 using 2-nitro-6,7,8,9-tetrahydropyrido[1,2-a]benzimidazole and 4′-(trifluoromethyl)[1,1′-biphenyl]-4-carboxylic acid, the title compound was obtained as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
c1ccn2c3c(nc2c1)CCCC3.c1ccccc1.c1ccccc1
Other
null
null
null
O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1.O=[N+]([O-])c1ccc2nc3c(n2c1)CCCC3>>O=C(Nc1ccc2nc3c(n2c1)CCCC3)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-67a716d4480145e18f502b905ad0f4c3
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1>>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cc4)cc3)cn12
C1(CC1)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1C.FC(C1=CC=C(C=C1)C1=CC=C(C=C1)C(=O)O)(F)F.Cl.C(C)(=O)OCC>>Cl.C1(CC1)C=1N=C2N(C=C(C=C2)NC(=O)C2=CC=C(C=C2)C2=CC=C(C=C2)C(F)(F)F)C1C
O=[N+:12]([O-])[c:11]1[cH:10][cH:9][c:8]2[n:7][c:3]([CH:4]3[CH2:5][CH2:6]3)[c:2]([CH3:1])[n:32]2[cH:31]1.O[C:13](=[O:14])[c:15]1[cH:16][cH:17][c:18](-[c:19]2[cH:20][cH:21][c:22]([C:23]([F:24])([F:25])[F:26])[cH:27][cH:28]2)[cH:29][cH:30]1>>[CH3:1][c:2]1[c:3]([CH:4]2[CH2:5][CH2:6]2)[n:7][c:8]2[cH:9][cH:10][c:11]([NH:12]...
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1
Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cc4)cc3)cn12
null
null
C(C)(=O)OCC
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ccc(-c2ccccc2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[N+;H0;D3:6](-[O-])-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
Operations similar to those of Example 1 were conducted using 2-cyclopropyl-3-methyl-6-nitroimidazo[1,2-a]pyridine and 4′-(trifluoromethyl)[1,1′-biphenyl]-4-carboxylic acid. The resulting solid was dissolved in ethyl acetate, followed by addition of 4N hydrochloric acid-ethyl acetate solution and concentration under re...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
C1CC1.c1ccn2ccnc2c1.c1ccccc1.c1ccccc1
Other
C(C)(=O)OCC
null
null
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1>C(C)(=O)OCC>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cc4)cc3)cn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-42e9fc4380bc4881991ed9fcabf600a7
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cn2)cc1>>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cn4)cc3)cn12
C1(CC1)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1C.FC(C=1C=CC(=NC1)C1=CC=C(C=C1)C(=O)O)(F)F.Cl.C(C)(=O)OCC>>Cl.C1(CC1)C=1N=C2N(C=C(C=C2)NC(C2=CC=C(C=C2)C2=NC=C(C=C2)C(F)(F)F)=O)C1C
O=[N+:12]([O-])[c:11]1[cH:10][cH:9][c:8]2[n:7][c:3]([CH:4]3[CH2:5][CH2:6]3)[c:2]([CH3:1])[n:32]2[cH:31]1.O[C:13](=[O:14])[c:15]1[cH:16][cH:17][c:18](-[c:19]2[cH:20][cH:21][c:22]([C:23]([F:24])([F:25])[F:26])[cH:27][n:28]2)[cH:29][cH:30]1>>[CH3:1][c:2]1[c:3]([CH:4]2[CH2:5][CH2:6]2)[n:7][c:8]2[cH:9][cH:10][c:11]([NH:12][...
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cn2)cc1
Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cn4)cc3)cn12
null
null
C(C)(=O)OCC
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ccc(-c2ccccn2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[N+;H0;D3:6](-[O-])-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
Operations similar to those of Example 1 were conducted using 2-cyclopropyl-3-methyl-6-nitroimidazo[1,2-a]pyridine and 4-[5-(trifluoromethyl)-2-pyridyl]benzenecarboxylic acid. The resulting solid was dissolved in ethyl acetate, followed by addition of 4N hydrochloric acid-ethyl acetate solution and concentration under ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
C1CC1.c1ccn2ccnc2c1.c1ccccc1.c1ccncc1
Other
C(C)(=O)OCC
null
null
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cn2)cc1>C(C)(=O)OCC>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cn4)cc3)cn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-471546c6ac364d7c96d3d1386dc55f67
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)(F)F)nc2)cc1>>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)nc4)cc3)cn12
C1(CC1)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1C.FC(C1=CC=C(C=N1)C1=CC=C(C=C1)C(=O)O)(F)F.Cl.C(C)(=O)OCC>>Cl.C1(CC1)C=1N=C2N(C=C(C=C2)NC(C2=CC=C(C=C2)C=2C=NC(=CC2)C(F)(F)F)=O)C1C
O=[N+:12]([O-])[c:11]1[cH:10][cH:9][c:8]2[n:7][c:3]([CH:4]3[CH2:5][CH2:6]3)[c:2]([CH3:1])[n:32]2[cH:31]1.O[C:13](=[O:14])[c:15]1[cH:16][cH:17][c:18](-[c:19]2[cH:20][cH:21][c:22]([C:23]([F:24])([F:25])[F:26])[n:27][cH:28]2)[cH:29][cH:30]1>>[CH3:1][c:2]1[c:3]([CH:4]2[CH2:5][CH2:6]2)[n:7][c:8]2[cH:9][cH:10][c:11]([NH:12][...
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)(F)F)nc2)cc1
Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)nc4)cc3)cn12
null
null
C(C)(=O)OCC
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ccc(-c2cccnc2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[N+;H0;D3:6](-[O-])-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
Operations similar to those of Example 1 were conducted using 2-cyclopropyl-3-methyl-6-nitroimidazo[1,2-a]pyridine and 4-[6-(trifluoromethyl)-3-pyridyl]benzenecarboxylic acid. The resulting solid was dissolved in ethyl acetate, followed by addition of 4N hydrochloric acid-ethyl acetate solution and concentration under ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
C1CC1.c1ccn2ccnc2c1.c1ccccc1.c1ccncc1
Other
C(C)(=O)OCC
null
null
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)(F)F)nc2)cc1>C(C)(=O)OCC>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)nc4)cc3)cn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-faeec0217aca4bbd90470800dbe0ea2c
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(F)nc2)cc1>>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(F)nc4)cc3)cn12
C1(CC1)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1C.FC1=CC=C(C=N1)C1=CC=C(C=C1)C(=O)O.Cl.C(C)(=O)OCC>>Cl.C1(CC1)C=1N=C2N(C=C(C=C2)NC(C2=CC=C(C=C2)C=2C=NC(=CC2)F)=O)C1C
O=[N+:12]([O-])[c:11]1[cH:10][cH:9][c:8]2[n:7][c:3]([CH:4]3[CH2:5][CH2:6]3)[c:2]([CH3:1])[n:29]2[cH:28]1.O[C:13](=[O:14])[c:15]1[cH:16][cH:17][c:18](-[c:19]2[cH:20][cH:21][c:22]([F:23])[n:24][cH:25]2)[cH:26][cH:27]1>>[CH3:1][c:2]1[c:3]([CH:4]2[CH2:5][CH2:6]2)[n:7][c:8]2[cH:9][cH:10][c:11]([NH:12][C:13](=[O:14])[c:15]3[...
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(F)nc2)cc1
Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(F)nc4)cc3)cn12
null
null
C(C)(=O)OCC
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ccc(-c2cccnc2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[N+;H0;D3:6](-[O-])-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
Operations similar to those of Example 1 were conducted using 2-cyclopropyl-3-methyl-6-nitroimidazo[1,2-a]pyridine and 4-(6-fluoro-3-pyridyl)benzenecarboxylic acid. The resulting solid was dissolved in ethyl acetate, followed by addition of 4N hydrochloric acid-ethyl acetate solution and concentration under reduced pre...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
C1CC1.c1ccn2ccnc2c1.c1ccccc1.c1ccncc1
Other
C(C)(=O)OCC
null
null
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(F)nc2)cc1>C(C)(=O)OCC>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(F)nc4)cc3)cn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ddfe61d417f14693b2cea5cbaec64845
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(Cl)cn2)cc1>>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(Cl)cn4)cc3)cn12
C1(CC1)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1C.ClC=1C=CC(=NC1)C1=CC=C(C=C1)C(=O)O>>ClC=1C=CC(=NC1)C1=CC=C(C(=O)NC=2C=CC=3N(C2)C(=C(N3)C3CC3)C)C=C1
O=[N+:12]([O-])[c:11]1[cH:10][cH:9][c:8]2[n:7][c:3]([CH:4]3[CH2:5][CH2:6]3)[c:2]([CH3:1])[n:29]2[cH:28]1.O[C:13](=[O:14])[c:15]1[cH:16][cH:17][c:18](-[c:19]2[cH:20][cH:21][c:22]([Cl:23])[cH:24][n:25]2)[cH:26][cH:27]1>>[CH3:1][c:2]1[c:3]([CH:4]2[CH2:5][CH2:6]2)[n:7][c:8]2[cH:9][cH:10][c:11]([NH:12][C:13](=[O:14])[c:15]3...
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(Cl)cn2)cc1
Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(Cl)cn4)cc3)cn12
null
null
null
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ccc(-c2ccccn2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[N+;H0;D3:6](-[O-])-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
Conducting the operations similar to those of Example 1 using 2-cyclopropyl-3-methyl-6-nitroimidazo[1,2-a]pyridine and 4-(5-chloro-2-pyridyl)benzenecarboxylic acid, the title compound was obtained as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
C1CC1.c1ccn2ccnc2c1.c1ccccc1.c1ccncc1
Other
null
null
null
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(Cl)cn2)cc1>>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(Cl)cn4)cc3)cn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-64c476b744b54932a8fec493085dd830
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ncc(-c2ccc(F)cc2)cn1>>Cc1c(C2CC2)nc2ccc(NC(=O)c3ncc(-c4ccc(F)cc4)cn3)cn12
C1(CC1)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1C.FC1=CC=C(C=C1)C=1C=NC(=NC1)C(=O)O.Cl.C(C)(=O)OCC>>Cl.C1(CC1)C=1N=C2N(C=C(C=C2)NC(=O)C2=NC=C(C=N2)C2=CC=C(C=C2)F)C1C
O=[N+:12]([O-])[c:11]1[cH:10][cH:9][c:8]2[n:7][c:3]([CH:4]3[CH2:5][CH2:6]3)[c:2]([CH3:1])[n:29]2[cH:28]1.O[C:13](=[O:14])[c:15]1[n:16][cH:17][c:18](-[c:19]2[cH:20][cH:21][c:22]([F:23])[cH:24][cH:25]2)[cH:26][n:27]1>>[CH3:1][c:2]1[c:3]([CH:4]2[CH2:5][CH2:6]2)[n:7][c:8]2[cH:9][cH:10][c:11]([NH:12][C:13](=[O:14])[c:15]3[n...
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ncc(-c2ccc(F)cc2)cn1
Cc1c(C2CC2)nc2ccc(NC(=O)c3ncc(-c4ccc(F)cc4)cn3)cn12
null
null
C(C)(=O)OCC
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ncc(-c2ccccc2)cn1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[#7;a:4]:[c:5]):[#7;a:6]:[c:7].O=[N+;H0;D3:8](-[O-])-[c:9](:[c:10]):[c:11]:[#7;a:12]1:[c:13]:[c:14]:[#7;a:15]:[c:16]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:8]-[c:9](:[c:10]):[c:11]:[#7;a:12]1:[c:13]:[c:14]:[#7;a:15]:[c:16]:1)-[c:3](:[#7;a:4]:[c:5]):[#7;a:6]:[c:7]
null
[]
null
null
null
null
2-cyclopropyl-3-methyl-6-nitroimidazo[1,2-a]pyridine and 5-(4-fluorophenyl)-2-pyrimidinecarboxylic acid. The resulting solid was dissolved in ethyl acetate, followed by addition of 4N hydrochloric acid-ethyl acetate solution and concentration under reduced pressure. The title compound was obtained as white solid. Condi...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
C1CC1.c1ccn2ccnc2c1.c1cncnc1.c1ccccc1
Other
C(C)(=O)OCC
null
null
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ncc(-c2ccc(F)cc2)cn1>C(C)(=O)OCC>Cc1c(C2CC2)nc2ccc(NC(=O)c3ncc(-c4ccc(F)cc4)cn3)cn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a7fa36e4a61548c682686ce652ecc4d0
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ncc(-c2cccc(F)c2)cn1>>Cc1c(C2CC2)nc2ccc(NC(=O)c3ncc(-c4cccc(F)c4)cn3)cn12
C1(CC1)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1C.FC=1C=C(C=CC1)C=1C=NC(=NC1)C(=O)O.Cl.C(C)(=O)OCC>>Cl.C1(CC1)C=1N=C2N(C=C(C=C2)NC(=O)C2=NC=C(C=N2)C2=CC(=CC=C2)F)C1C
O=[N+:12]([O-])[c:11]1[cH:10][cH:9][c:8]2[n:7][c:3]([CH:4]3[CH2:5][CH2:6]3)[c:2]([CH3:1])[n:29]2[cH:28]1.O[C:13](=[O:14])[c:15]1[n:16][cH:17][c:18](-[c:19]2[cH:20][cH:21][cH:22][c:23]([F:24])[cH:25]2)[cH:26][n:27]1>>[CH3:1][c:2]1[c:3]([CH:4]2[CH2:5][CH2:6]2)[n:7][c:8]2[cH:9][cH:10][c:11]([NH:12][C:13](=[O:14])[c:15]3[n...
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ncc(-c2cccc(F)c2)cn1
Cc1c(C2CC2)nc2ccc(NC(=O)c3ncc(-c4cccc(F)c4)cn3)cn12
null
null
C(C)(=O)OCC
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ncc(-c2ccccc2)cn1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[#7;a:4]:[c:5]):[#7;a:6]:[c:7].O=[N+;H0;D3:8](-[O-])-[c:9](:[c:10]):[c:11]:[#7;a:12]1:[c:13]:[c:14]:[#7;a:15]:[c:16]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:8]-[c:9](:[c:10]):[c:11]:[#7;a:12]1:[c:13]:[c:14]:[#7;a:15]:[c:16]:1)-[c:3](:[#7;a:4]:[c:5]):[#7;a:6]:[c:7]
null
[]
null
null
null
null
Operations similar to those of Example 1 were conducted using 2-cyclopropyl-3-methyl-6-nitroimidazo[1,2-a]pyridine and 5-(3-fluorophenyl)-2-pyrimidinecarboxylic acid. The resulting solid was dissolved in ethyl acetate, followed by addition of 4N hydrochloric acid-ethyl acetate solution and concentration under reduced p...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
C1CC1.c1ccn2ccnc2c1.c1cncnc1.c1ccccc1
Other
C(C)(=O)OCC
null
null
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ncc(-c2cccc(F)c2)cn1>C(C)(=O)OCC>Cc1c(C2CC2)nc2ccc(NC(=O)c3ncc(-c4cccc(F)c4)cn3)cn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5893d9713992467291546c5e764751aa
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1cnc(-c2ccc(F)cc2)cn1>>Cc1c(C2CC2)nc2ccc(NC(=O)c3cnc(-c4ccc(F)cc4)cn3)cn12
C1(CC1)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1C.FC1=CC=C(C=C1)C=1N=CC(=NC1)C(=O)O.Cl.C(C)(=O)OCC>>Cl.C1(CC1)C=1N=C2N(C=C(C=C2)NC(=O)C2=NC=C(N=C2)C2=CC=C(C=C2)F)C1C
O=[N+:12]([O-])[c:11]1[cH:10][cH:9][c:8]2[n:7][c:3]([CH:4]3[CH2:5][CH2:6]3)[c:2]([CH3:1])[n:29]2[cH:28]1.O[C:13](=[O:14])[c:15]1[cH:16][n:17][c:18](-[c:19]2[cH:20][cH:21][c:22]([F:23])[cH:24][cH:25]2)[cH:26][n:27]1>>[CH3:1][c:2]1[c:3]([CH:4]2[CH2:5][CH2:6]2)[n:7][c:8]2[cH:9][cH:10][c:11]([NH:12][C:13](=[O:14])[c:15]3[c...
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1cnc(-c2ccc(F)cc2)cn1
Cc1c(C2CC2)nc2ccc(NC(=O)c3cnc(-c4ccc(F)cc4)cn3)cn12
null
null
C(C)(=O)OCC
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nc(C3CC3)cn2c1)c1cnc(-c2ccccc2)cn1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#7;a:4]:[c:5]:[c:6]:[#7;a:7]:[c:8]:1.O=[N+;H0;D3:9](-[O-])-[c:10](:[c:11]):[c:12]:[#7;a:13]1:[c:14]:[c:15]:[#7;a:16]:[c:17]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:9]-[c:10](:[c:11]):[c:12]:[#7;a:13]1:[c:14]:[c:15]:[#7;a:16]:[c:17]:1)-[c:3]1:[#7;a:4]:[c:5]:[c:6]:[#7;a:7]:[c:8]:1
null
[]
null
null
null
null
Operations similar to those of Example 1 were conducted using 2-cyclopropyl-3-methyl-6-nitroimidazo[1,2-a]pyridine and 5-(4-fluorophenyl)-2-pyrazinecarboxylic acid. The resulting solid was dissolved in ethyl acetate, followed by addition of 4N hydrochloric acid-ethyl acetate solution and concentration under reduced pre...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
C1CC1.c1ccn2ccnc2c1.c1cnccn1.c1ccccc1
Other
C(C)(=O)OCC
null
null
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1cnc(-c2ccc(F)cc2)cn1>C(C)(=O)OCC>Cc1c(C2CC2)nc2ccc(NC(=O)c3cnc(-c4ccc(F)cc4)cn3)cn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3ac85a5ef6bb47a99958880427975d44
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(F)cc2)cn1>>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(F)cc4)cn3)cn12
C1(CC1)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1C.FC1=CC=C(C=C1)C=1C=CC(=NC1)C(=O)O.Cl.C(C)(=O)OCC>>Cl.C1(CC1)C=1N=C2N(C=C(C=C2)NC(=O)C2=NC=C(C=C2)C2=CC=C(C=C2)F)C1C
O=[N+:12]([O-])[c:11]1[cH:10][cH:9][c:8]2[n:7][c:3]([CH:4]3[CH2:5][CH2:6]3)[c:2]([CH3:1])[n:29]2[cH:28]1.O[C:13](=[O:14])[c:15]1[cH:16][cH:17][c:18](-[c:19]2[cH:20][cH:21][c:22]([F:23])[cH:24][cH:25]2)[cH:26][n:27]1>>[CH3:1][c:2]1[c:3]([CH:4]2[CH2:5][CH2:6]2)[n:7][c:8]2[cH:9][cH:10][c:11]([NH:12][C:13](=[O:14])[c:15]3[...
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(F)cc2)cn1
Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(F)cc4)cn3)cn12
null
null
C(C)(=O)OCC
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ccc(-c2ccccc2)cn1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#7;a:5]:[c:6].O=[N+;H0;D3:7](-[O-])-[c:8](:[c:9]):[c:10]:[#7;a:11]1:[c:12]:[c:13]:[#7;a:14]:[c:15]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:7]-[c:8](:[c:9]):[c:10]:[#7;a:11]1:[c:12]:[c:13]:[#7;a:14]:[c:15]:1)-[c:3](:[c:4]):[#7;a:5]:[c:6]
null
[]
null
null
null
null
Operations similar to those of Example 1 were conducted using 2-cyclopropyl-3-methyl-6-nitroimidazo[1,2-a]pyridine and 5-(4-fluorophenyl)-2-pyridinecarboxylic acid. The resulting solid was dissolved in ethyl acetate, followed by addition of 4N hydrochloric acid-ethyl acetate solution and concentration under reduced pre...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
C1CC1.c1ccn2ccnc2c1.c1ccncc1.c1ccccc1
Other
C(C)(=O)OCC
null
null
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(F)cc2)cn1>C(C)(=O)OCC>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(F)cc4)cn3)cn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d3d8e3b51cb34b638d44b7ce49ebfd54
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(F)cc2)nc1>>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(F)cc4)nc3)cn12
C1(CC1)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1C.FC1=CC=C(C=C1)C1=NC=C(C(=O)O)C=C1.Cl.C(C)(=O)OCC>>Cl.C1(CC1)C=1N=C2N(C=C(C=C2)NC(C2=CN=C(C=C2)C2=CC=C(C=C2)F)=O)C1C
O=[N+:12]([O-])[c:11]1[cH:10][cH:9][c:8]2[n:7][c:3]([CH:4]3[CH2:5][CH2:6]3)[c:2]([CH3:1])[n:29]2[cH:28]1.O[C:13](=[O:14])[c:15]1[cH:16][cH:17][c:18](-[c:19]2[cH:20][cH:21][c:22]([F:23])[cH:24][cH:25]2)[n:26][cH:27]1>>[CH3:1][c:2]1[c:3]([CH:4]2[CH2:5][CH2:6]2)[n:7][c:8]2[cH:9][cH:10][c:11]([NH:12][C:13](=[O:14])[c:15]3[...
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(F)cc2)nc1
Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(F)cc4)nc3)cn12
null
null
C(C)(=O)OCC
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ccc(-c2ccccc2)nc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]:[#7;a:6]:[c:7].O=[N+;H0;D3:8](-[O-])-[c:9](:[c:10]):[c:11]:[#7;a:12]1:[c:13]:[c:14]:[#7;a:15]:[c:16]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:8]-[c:9](:[c:10]):[c:11]:[#7;a:12]1:[c:13]:[c:14]:[#7;a:15]:[c:16]:1)-[c:3](:[c:4]):[c:5]:[#7;a:6]:[c:7]
null
[]
null
null
null
null
Operations similar to those of Example 1 were conducted using 2-cyclopropyl-3-methyl-6-nitroimidazo[1,2-a]pyridine and 6-(4-fluorophenyl)nicotinic acid. The resulting solid was dissolved in ethyl acetate, followed by addition of 4N hydrochloric acid-ethyl acetate solution and concentration under reduced pressure. The t...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
C1CC1.c1ccn2ccnc2c1.c1ccncc1.c1ccccc1
Other
C(C)(=O)OCC
null
null
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(F)cc2)nc1>C(C)(=O)OCC>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(F)cc4)nc3)cn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-78f3a0969f734ff0bb0c3bcd6300676e
Cc1c(C2CCOC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cn2)cc1>>Cc1c(C2CCOC2)nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cn4)cc3)cn12
CC1=C(N=C2N1C=C(C=C2)[N+](=O)[O-])C2COCC2.FC(C=1C=CC(=NC1)C1=CC=C(C=C1)C(=O)O)(F)F>>CC1=C(N=C2N1C=C(C=C2)NC(C2=CC=C(C=C2)C2=NC=C(C=C2)C(F)(F)F)=O)C2COCC2
O=[N+:14]([O-])[c:13]1[cH:12][cH:11][c:10]2[n:9][c:3]([CH:4]3[CH2:5][CH2:6][O:7][CH2:8]3)[c:2]([CH3:1])[n:34]2[cH:33]1.O[C:15](=[O:16])[c:17]1[cH:18][cH:19][c:20](-[c:21]2[cH:22][cH:23][c:24]([C:25]([F:26])([F:27])[F:28])[cH:29][n:30]2)[cH:31][cH:32]1>>[CH3:1][c:2]1[c:3]([CH:4]2[CH2:5][CH2:6][O:7][CH2:8]2)[n:9][c:10]2[...
Cc1c(C2CCOC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cn2)cc1
Cc1c(C2CCOC2)nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cn4)cc3)cn12
null
null
null
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nc(C3CCOC3)cn2c1)c1ccc(-c2ccccn2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[N+;H0;D3:6](-[O-])-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[#7;a:12]:[c:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[#7;a:12]:[c:13]:[c:14]:1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
Conducting the operations similar to those of Example 1 using 3-methyl-6-nitro-2-tetrahydro-3-furanylimidazo[1,2-a]pyridine and 4-[5-(trifluoromethyl)-2-pyridyl]benzenecarboxylic acid, the title compound was obtained as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
C1CCOC1.c1ccn2ccnc2c1.c1ccccc1.c1ccncc1
Other
null
null
null
Cc1c(C2CCOC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cn2)cc1>>Cc1c(C2CCOC2)nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cn4)cc3)cn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5705660825af490f91854d7019e6ba9d
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccccn2)cc1>>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccccn4)cc3)cn12
C1(CC1)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1C.N1=C(C=CC=C1)C1=CC=C(C=C1)C(=O)O.Cl.C(C)(=O)OCC>>Cl.C1(CC1)C=1N=C2N(C=C(C=C2)NC(C2=CC=C(C=C2)C2=NC=CC=C2)=O)C1C
O=[N+:12]([O-])[c:11]1[cH:10][cH:9][c:8]2[n:7][c:3]([CH:4]3[CH2:5][CH2:6]3)[c:2]([CH3:1])[n:28]2[cH:27]1.O[C:13](=[O:14])[c:15]1[cH:16][cH:17][c:18](-[c:19]2[cH:20][cH:21][cH:22][cH:23][n:24]2)[cH:25][cH:26]1>>[CH3:1][c:2]1[c:3]([CH:4]2[CH2:5][CH2:6]2)[n:7][c:8]2[cH:9][cH:10][c:11]([NH:12][C:13](=[O:14])[c:15]3[cH:16][...
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccccn2)cc1
Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccccn4)cc3)cn12
null
null
C(C)(=O)OCC
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ccc(-c2ccccn2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[N+;H0;D3:6](-[O-])-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
The title compound was obtained as white solid by conducting the operations similar to those of Example 1, using 2-cyclopropyl-3-methyl-6-nitroimidazo[1,2-a]pyridine and 4-(2-pyridyl)benzenecarboxylic acid. The resulting solid was dissolved in ethyl acetate, followed by addition of 4N hydrochloric acid-ethyl acetate so...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
C1CC1.c1ccn2ccnc2c1.c1ccccc1.c1ccncc1
Other
C(C)(=O)OCC
null
null
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccccn2)cc1>C(C)(=O)OCC>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccccn4)cc3)cn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-68a0db620496425fa19765d6d6a62c4a
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)CCc1ccc(C(F)(F)F)cc1>>Cc1c(C2CC2)nc2ccc(NC(=O)CCc3ccc(C(F)(F)F)cc3)cn12
C1(CC1)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1C.FC(C1=CC=C(C=C1)CCC(=O)O)(F)F>>C1(CC1)C=1N=C2N(C=C(C=C2)NC(CCC2=CC=C(C=C2)C(F)(F)F)=O)C1C
O=[N+:12]([O-])[c:11]1[cH:10][cH:9][c:8]2[n:7][c:3]([CH:4]3[CH2:5][CH2:6]3)[c:2]([CH3:1])[n:28]2[cH:27]1.O[C:13](=[O:14])[CH2:15][CH2:16][c:17]1[cH:18][cH:19][c:20]([C:21]([F:22])([F:23])[F:24])[cH:25][cH:26]1>>[CH3:1][c:2]1[c:3]([CH:4]2[CH2:5][CH2:6]2)[n:7][c:8]2[cH:9][cH:10][c:11]([NH:12][C:13](=[O:14])[CH2:15][CH2:1...
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)CCc1ccc(C(F)(F)F)cc1
Cc1c(C2CC2)nc2ccc(NC(=O)CCc3ccc(C(F)(F)F)cc3)cn12
null
null
null
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(CCc1ccccc1)Nc1ccc2nc(C3CC3)cn2c1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4].O=[N+;H0;D3:5](-[O-])-[c:6](:[c:7]):[c:8]:[#7;a:9]1:[c:10]:[c:11]:[#7;a:12]:[c:13]:1>>[C:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:5]-[c:6](:[c:7]):[c:8]:[#7;a:9]1:[c:10]:[c:11]:[#7;a:12]:[c:13]:1
null
[]
null
null
null
null
Conducting the operations similar to those of Example 1 using 2-cyclopropyl-3-methyl-6-nitroimidazo[1,2-a]pyridine and 3-[4-(trifluoromethyl)phenyl]propionic acid, the title compound was obtained as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
C1CC1.c1ccn2ccnc2c1.c1ccccc1
Other
null
null
null
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)CCc1ccc(C(F)(F)F)cc1>>Cc1c(C2CC2)nc2ccc(NC(=O)CCc3ccc(C(F)(F)F)cc3)cn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4d92e00a2dc54f048bb7884db64f9ae2
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)CCc1ccc(C(F)(F)F)nc1>>Cc1c(C2CC2)nc2ccc(NC(=O)CCc3ccc(C(F)(F)F)nc3)cn12
C1(CC1)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1C.FC(C1=CC=C(C=N1)CCC(=O)O)(F)F>>C1(CC1)C=1N=C2N(C=C(C=C2)NC(CCC=2C=NC(=CC2)C(F)(F)F)=O)C1C
O=[N+:12]([O-])[c:11]1[cH:10][cH:9][c:8]2[n:7][c:3]([CH:4]3[CH2:5][CH2:6]3)[c:2]([CH3:1])[n:28]2[cH:27]1.O[C:13](=[O:14])[CH2:15][CH2:16][c:17]1[cH:18][cH:19][c:20]([C:21]([F:22])([F:23])[F:24])[n:25][cH:26]1>>[CH3:1][c:2]1[c:3]([CH:4]2[CH2:5][CH2:6]2)[n:7][c:8]2[cH:9][cH:10][c:11]([NH:12][C:13](=[O:14])[CH2:15][CH2:16...
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)CCc1ccc(C(F)(F)F)nc1
Cc1c(C2CC2)nc2ccc(NC(=O)CCc3ccc(C(F)(F)F)nc3)cn12
null
null
null
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(CCc1cccnc1)Nc1ccc2nc(C3CC3)cn2c1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4].O=[N+;H0;D3:5](-[O-])-[c:6](:[c:7]):[c:8]:[#7;a:9]1:[c:10]:[c:11]:[#7;a:12]:[c:13]:1>>[C:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:5]-[c:6](:[c:7]):[c:8]:[#7;a:9]1:[c:10]:[c:11]:[#7;a:12]:[c:13]:1
null
[]
null
null
null
null
Conducting the operations similar to those of Example 1 using 2-cyclopropyl-3-methyl-6-nitroimidazo[1,2-a]pyridine and 3-[6-(trifluoromethyl)-3-pyridyl]propionic acid, the title compound was obtained as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
C1CC1.c1ccn2ccnc2c1.c1ccncc1
Other
null
null
null
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)CCc1ccc(C(F)(F)F)nc1>>Cc1c(C2CC2)nc2ccc(NC(=O)CCc3ccc(C(F)(F)F)nc3)cn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-cee137feb6da4ccf9328aa7dec8e873c
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(OC(F)F)cn2)cc1>>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(OC(F)F)cn4)cc3)cn12
C1(CC1)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1C.FC(OC=1C=CC(=NC1)C1=CC=C(C=C1)C(=O)O)F>>C1(CC1)C=1N=C2N(C=C(C=C2)NC(C2=CC=C(C=C2)C2=NC=C(C=C2)OC(F)F)=O)C1C
O=[N+:12]([O-])[c:11]1[cH:10][cH:9][c:8]2[n:7][c:3]([CH:4]3[CH2:5][CH2:6]3)[c:2]([CH3:1])[n:32]2[cH:31]1.O[C:13](=[O:14])[c:15]1[cH:16][cH:17][c:18](-[c:19]2[cH:20][cH:21][c:22]([O:23][CH:24]([F:25])[F:26])[cH:27][n:28]2)[cH:29][cH:30]1>>[CH3:1][c:2]1[c:3]([CH:4]2[CH2:5][CH2:6]2)[n:7][c:8]2[cH:9][cH:10][c:11]([NH:12][C...
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(OC(F)F)cn2)cc1
Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(OC(F)F)cn4)cc3)cn12
null
null
null
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ccc(-c2ccccn2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[N+;H0;D3:6](-[O-])-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
Conducting the operations similar to those of Example 1 using 2-cyclopropyl-3-methyl-6-nitroimidazo[1,2-a]pyridine and 4-[5-(difluoromethoxy)-2-pyridyl]benzenecarboxylic acid, the title compound was obtained as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
C1CC1.c1ccn2ccnc2c1.c1ccccc1.c1ccncc1
Other
null
null
null
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(OC(F)F)cn2)cc1>>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(OC(F)F)cn4)cc3)cn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f1e9d625d2be4c0bb5d8523a66c12da0
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)F)nc2)cc1>>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)F)nc4)cc3)cn12
C1(CC1)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1C.FC(C1=CC=C(C=N1)C1=CC=C(C=C1)C(=O)O)F>>C1(CC1)C=1N=C2N(C=C(C=C2)NC(C2=CC=C(C=C2)C=2C=NC(=CC2)C(F)F)=O)C1C
O=[N+:12]([O-])[c:11]1[cH:10][cH:9][c:8]2[n:7][c:3]([CH:4]3[CH2:5][CH2:6]3)[c:2]([CH3:1])[n:31]2[cH:30]1.O[C:13](=[O:14])[c:15]1[cH:16][cH:17][c:18](-[c:19]2[cH:20][cH:21][c:22]([CH:23]([F:24])[F:25])[n:26][cH:27]2)[cH:28][cH:29]1>>[CH3:1][c:2]1[c:3]([CH:4]2[CH2:5][CH2:6]2)[n:7][c:8]2[cH:9][cH:10][c:11]([NH:12][C:13](=...
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)F)nc2)cc1
Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)F)nc4)cc3)cn12
null
null
null
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ccc(-c2cccnc2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[N+;H0;D3:6](-[O-])-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
Conducting the operations similar to those of Example 1 using 2-cyclopropyl-3-methyl-6-nitroimidazo[1,2-a]pyridine and 4-[6-(difluoromethyl)-3-pyridyl]benzenecarboxylic acid, the title compound was obtained as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
C1CC1.c1ccn2ccnc2c1.c1ccccc1.c1ccncc1
Other
null
null
null
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)F)nc2)cc1>>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)F)nc4)cc3)cn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b566a84903c24897bebab23fb36e3eff
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1F>>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cc4)cc3F)cn12
C1(CC1)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1C.FC=1C=C(C=CC1C(=O)O)C1=CC=C(C=C1)C(F)(F)F>>C1(CC1)C=1N=C2N(C=C(C=C2)NC(=O)C2=C(C=C(C=C2)C2=CC=C(C=C2)C(F)(F)F)F)C1C
O=[N+:12]([O-])[c:11]1[cH:10][cH:9][c:8]2[n:7][c:3]([CH:4]3[CH2:5][CH2:6]3)[c:2]([CH3:1])[n:33]2[cH:32]1.O[C:13](=[O:14])[c:15]1[cH:16][cH:17][c:18](-[c:19]2[cH:20][cH:21][c:22]([C:23]([F:24])([F:25])[F:26])[cH:27][cH:28]2)[cH:29][c:30]1[F:31]>>[CH3:1][c:2]1[c:3]([CH:4]2[CH2:5][CH2:6]2)[n:7][c:8]2[cH:9][cH:10][c:11]([N...
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1F
Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cc4)cc3F)cn12
null
null
null
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ccc(-c2ccccc2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[N+;H0;D3:6](-[O-])-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
Conducting the operations similar to those of Example 1 using 2-cyclopropyl-3-methyl-6-nitroimidazo[1,2-a]pyridine and 3-fluoro-4′-(trifluoromethyl)[1,1′-biphenyl]-4-carboxylic acid, the title compound was obtained as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
C1CC1.c1ccn2ccnc2c1.c1ccccc1.c1ccccc1
Other
null
null
null
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1F>>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cc4)cc3F)cn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b05bc350b84b43b582635aa0845d7bf0
CS(=O)(=O)c1ccc(-c2ccc(C(=O)O)cc2)cc1.Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12>>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(S(C)(=O)=O)cc4)cc3)cn12
C1(CC1)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1C.CS(=O)(=O)C1=CC=C(C=C1)C1=CC=C(C=C1)C(=O)O>>C1(CC1)C=1N=C2N(C=C(C=C2)NC(=O)C2=CC=C(C=C2)C2=CC=C(C=C2)S(=O)(=O)C)C1C
O[C:13](=[O:14])[c:15]1[cH:16][cH:17][c:18](-[c:19]2[cH:20][cH:21][c:22]([S:23]([CH3:24])(=[O:25])=[O:26])[cH:27][cH:28]2)[cH:29][cH:30]1.O=[N+:12]([O-])[c:11]1[cH:10][cH:9][c:8]2[n:7][c:3]([CH:4]3[CH2:5][CH2:6]3)[c:2]([CH3:1])[n:32]2[cH:31]1>>[CH3:1][c:2]1[c:3]([CH:4]2[CH2:5][CH2:6]2)[n:7][c:8]2[cH:9][cH:10][c:11]([NH...
CS(=O)(=O)c1ccc(-c2ccc(C(=O)O)cc2)cc1.Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12
Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(S(C)(=O)=O)cc4)cc3)cn12
null
null
null
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ccc(-c2ccccc2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[N+;H0;D3:6](-[O-])-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
Conducting the operations similar to those of Example 1 using 2-cyclopropyl-3-methyl-6-nitroimidazo[1,2-a]pyridine and 4′-(methylsulfonyl)[1,1′-biphenyl]-4-carboxylic acid, the title compound was obtained as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
C1CC1.c1ccn2ccnc2c1.c1ccccc1.c1ccccc1
Other
null
null
null
CS(=O)(=O)c1ccc(-c2ccc(C(=O)O)cc2)cc1.Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12>>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(S(C)(=O)=O)cc4)cc3)cn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-535d476dad0143fa8e4b3d3235b1f036
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(Cl)nn2)cc1>>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(Cl)nn4)cc3)cn12
C1(CC1)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1C.ClC1=CC=C(N=N1)C1=CC=C(C=C1)C(=O)O>>ClC1=CC=C(N=N1)C1=CC=C(C(=O)NC=2C=CC=3N(C2)C(=C(N3)C3CC3)C)C=C1
O=[N+:12]([O-])[c:11]1[cH:10][cH:9][c:8]2[n:7][c:3]([CH:4]3[CH2:5][CH2:6]3)[c:2]([CH3:1])[n:29]2[cH:28]1.O[C:13](=[O:14])[c:15]1[cH:16][cH:17][c:18](-[c:19]2[cH:20][cH:21][c:22]([Cl:23])[n:24][n:25]2)[cH:26][cH:27]1>>[CH3:1][c:2]1[c:3]([CH:4]2[CH2:5][CH2:6]2)[n:7][c:8]2[cH:9][cH:10][c:11]([NH:12][C:13](=[O:14])[c:15]3[...
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(Cl)nn2)cc1
Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(Cl)nn4)cc3)cn12
null
null
null
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ccc(-c2cccnn2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[N+;H0;D3:6](-[O-])-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
Operations similar to Example 1 were conducted using 2-cyclopropyl-3-methyl-6-nitroimidazo[1,2-a]pyridine and 4-(6-chloro-3-pyridazinyl)benzenecarboxylic acid, to provide the title compound as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
C1CC1.c1ccn2ccnc2c1.c1ccccc1.c1ccnnc1
Other
null
null
null
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(Cl)nn2)cc1>>Cc1c(C2CC2)nc2ccc(NC(=O)c3ccc(-c4ccc(Cl)nn4)cc3)cn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-617b41c59b904c528d3936db5b9d1ae4
COc1ccc(-c2ccc(C(=O)O)cc2)nc1.Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12>>COc1ccc(-c2ccc(C(=O)Nc3ccc4nc(C5CC5)c(C)n4c3)cc2)nc1
C1(CC1)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1C.COC=1C=CC(=NC1)C1=CC=C(C=C1)C(=O)O>>C1(CC1)C=1N=C2N(C=C(C=C2)NC(C2=CC=C(C=C2)C2=NC=C(C=C2)OC)=O)C1C
O[C:11]([c:10]1[cH:9][cH:8][c:7](-[c:6]2[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:30][n:29]2)[cH:28][cH:27]1)=[O:12].O=[N+:13]([O-])[c:14]1[cH:15][cH:16][c:17]2[n:18][c:19]([CH:20]3[CH2:21][CH2:22]3)[c:23]([CH3:24])[n:25]2[cH:26]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([C:11](=[O:12])[NH:13][c:14]3[cH:...
COc1ccc(-c2ccc(C(=O)O)cc2)nc1.Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12
COc1ccc(-c2ccc(C(=O)Nc3ccc4nc(C5CC5)c(C)n4c3)cc2)nc1
null
null
null
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ccc(-c2ccccn2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[N+;H0;D3:6](-[O-])-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[#7;a:12]:[c:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[#7;a:12]:[c:13]:[c:14]:1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
Operations similar to Example 1 were conducted using 2-cyclopropyl-3-methyl-6-nitroimidazo[1,2-a]pyridine and 4-(5-methoxy-2-pyridyl)benzenecarboxylic acid, to provide the title compound as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
c1ccncc1.c1ccccc1.c1ccn2ccnc2c1.C1CC1
Other
null
null
null
COc1ccc(-c2ccc(C(=O)O)cc2)nc1.Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12>>COc1ccc(-c2ccc(C(=O)Nc3ccc4nc(C5CC5)c(C)n4c3)cc2)nc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-936628b1b56b4a2fa90f81010c84e676
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.Cc1ccc(-c2ccc(C(=O)O)cc2)nc1>>Cc1ccc(-c2ccc(C(=O)Nc3ccc4nc(C5CC5)c(C)n4c3)cc2)nc1
C1(CC1)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1C.CC=1C=CC(=NC1)C1=CC=C(C=C1)C(=O)O>>C1(CC1)C=1N=C2N(C=C(C=C2)NC(C2=CC=C(C=C2)C2=NC=C(C=C2)C)=O)C1C
O=[N+:12]([O-])[c:13]1[cH:14][cH:15][c:16]2[n:17][c:18]([CH:19]3[CH2:20][CH2:21]3)[c:22]([CH3:23])[n:24]2[cH:25]1.O[C:10]([c:9]1[cH:8][cH:7][c:6](-[c:5]2[cH:4][cH:3][c:2]([CH3:1])[cH:29][n:28]2)[cH:27][cH:26]1)=[O:11]>>[CH3:1][c:2]1[cH:3][cH:4][c:5](-[c:6]2[cH:7][cH:8][c:9]([C:10](=[O:11])[NH:12][c:13]3[cH:14][cH:15][c...
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.Cc1ccc(-c2ccc(C(=O)O)cc2)nc1
Cc1ccc(-c2ccc(C(=O)Nc3ccc4nc(C5CC5)c(C)n4c3)cc2)nc1
null
null
null
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ccc(-c2ccccn2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[N+;H0;D3:6](-[O-])-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[#7;a:12]:[c:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[#7;a:12]:[c:13]:[c:14]:1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
Operations similar to Example 1 were conducted using 2-cyclopropyl-3-methyl-6-nitroimidazo[1,2-a]pyridine and 4-(5-methyl-2-pyridyl)benzenecarboxylic acid, to provide the title compound as white solid. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
c1ccncc1.c1ccccc1.c1ccn2ccnc2c1.C1CC1
Other
null
null
null
Cc1c(C2CC2)nc2ccc([N+](=O)[O-])cn12.Cc1ccc(-c2ccc(C(=O)O)cc2)nc1>>Cc1ccc(-c2ccc(C(=O)Nc3ccc4nc(C5CC5)c(C)n4c3)cc2)nc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7374e82fce514343986cd10121234652
CCOC(=O)c1cn2cc([N+](=O)[O-])ccc2n1.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1>>CCOC(=O)c1cn2cc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cc4)cc3)ccc2n1
[N+](=O)([O-])C=1C=CC=2N(C1)C=C(N2)C(=O)OCC.FC(C1=CC=C(C=C1)C1=CC=C(C=C1)C(=O)O)(F)F>>FC(C1=CC=C(C=C1)C1=CC=C(C=C1)C(=O)NC=1C=CC=2N(C1)C=C(N2)C(=O)OCC)(F)F
O=[N+:11]([O-])[c:10]1[cH:9][n:8]2[cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[n:33][c:32]2[cH:31][cH:30]1.O[C:12](=[O:13])[c:14]1[cH:15][cH:16][c:17](-[c:18]2[cH:19][cH:20][c:21]([C:22]([F:23])([F:24])[F:25])[cH:26][cH:27]2)[cH:28][cH:29]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][n:8]2[cH:9][c:10]([NH:11][C:12](...
CCOC(=O)c1cn2cc([N+](=O)[O-])ccc2n1.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1
CCOC(=O)c1cn2cc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cc4)cc3)ccc2n1
null
null
null
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nccn2c1)c1ccc(-c2ccccc2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[N+;H0;D3:6](-[O-])-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[#7;a:12]:[c:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[#7;a:12]:[c:13]:[c:14]:1)-[c:3](:[c:4]):[c:5]
31.1
[{"value": 31.1, "product": "FC(C1=CC=C(C=C1)C1=CC=C(C=C1)C(=O)NC=1C=CC=2N(C1)C=C(N2)C(=O)OCC)(F)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Operations similar to Example 1 were conducted using ethyl 6-nitroimidazo[1,2-a]pyridine-2-carboxylate (600 mg) and 4′-(trifluoromethyl)[1,1′-biphenyl]-4-carboxylic acid (700 mg), to provide ethyl 6-({[4′-(trifluoromethyl)[1,1′-biphenyl]-4-yl]carbonyl}-amino)imidazo[1,2-a]pyridine-2-carboxylate (360 mg) as white solid....
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
c1ccn2ccnc2c1.c1ccccc1.c1ccccc1
Other
null
null
null
CCOC(=O)c1cn2cc([N+](=O)[O-])ccc2n1.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1>>CCOC(=O)c1cn2cc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cc4)cc3)ccc2n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-35e34d64bc5c4d9e8fe81e0963413302
COC(=O)c1nc2ccc([N+](=O)[O-])cn2c1C.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1>>COC(=O)c1nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cc4)cc3)cn2c1C
CC1=C(N=C2N1C=C(C=C2)[N+](=O)[O-])C(=O)OC.FC(C1=CC=C(C=C1)C1=CC=C(C=C1)C(=O)O)(F)F>>CC1=C(N=C2N1C=C(C=C2)NC(=O)C2=CC=C(C=C2)C2=CC=C(C=C2)C(F)(F)F)C(=O)OC
O=[N+:11]([O-])[c:10]1[cH:9][cH:8][c:7]2[n:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[c:32]([CH3:33])[n:31]2[cH:30]1.O[C:12](=[O:13])[c:14]1[cH:15][cH:16][c:17](-[c:18]2[cH:19][cH:20][c:21]([C:22]([F:23])([F:24])[F:25])[cH:26][cH:27]2)[cH:28][cH:29]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[n:6][c:7]2[cH:8][cH:9][c:10]([NH:11][C:12](=...
COC(=O)c1nc2ccc([N+](=O)[O-])cn2c1C.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1
COC(=O)c1nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cc4)cc3)cn2c1C
null
null
null
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nccn2c1)c1ccc(-c2ccccc2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[N+;H0;D3:6](-[O-])-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
Operations similar to those of Example 1 were conducted using methyl 3-methyl-6-nitroimidazo[1,2-a]pyridine-2-carboxylate and 4′-(trifluoromethyl)[1,1′-biphenyl]-4-carboxylic acid, to provide methyl 3-methyl-6-({[4′-(trifluoromethyl)[1,1′-biphenyl]-4-yl]-carbonyl}amino)-imidazo[1,2-a]pyridine-2-carboxylate as white sol...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
c1ccn2ccnc2c1.c1ccccc1.c1ccccc1
Other
null
null
null
COC(=O)c1nc2ccc([N+](=O)[O-])cn2c1C.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1>>COC(=O)c1nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cc4)cc3)cn2c1C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c68a44aad67a41719d3f49522f7f6d59
O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1.O=[N+]([O-])c1ccc2nc(C3CC3)cn2c1>>O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1
Br.C1(CC1)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1.FC(C1=CC=C(C=C1)C1=CC=C(C=C1)C(=O)O)(F)F>>C1(CC1)C=1N=C2N(C=C(C=C2)NC(=O)C2=CC=C(C=C2)C2=CC=C(C=C2)C(F)(F)F)C1
O[C:2](=[O:1])[c:16]1[cH:17][cH:18][c:19](-[c:20]2[cH:21][cH:22][c:23]([C:24]([F:25])([F:26])[F:27])[cH:28][cH:29]2)[cH:30][cH:31]1.O=[N+:3]([O-])[c:4]1[cH:5][cH:6][c:7]2[n:8][c:9]([CH:10]3[CH2:11][CH2:12]3)[cH:13][n:14]2[cH:15]1>>[O:1]=[C:2]([NH:3][c:4]1[cH:5][cH:6][c:7]2[n:8][c:9]([CH:10]3[CH2:11][CH2:12]3)[cH:13][n:...
O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1.O=[N+]([O-])c1ccc2nc(C3CC3)cn2c1
O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1
null
null
null
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ccc(-c2ccccc2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[N+;H0;D3:6](-[O-])-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
Operations similar to those of Example 1 were conducted using 2-cyclopropyl-6-nitroimidazo[1,2-a]pyridine hydrobromide and 4′-(trifluoromethyl)[1,1′-biphenyl]-4-carboxylic acid, to provide N-(2-cyclopropylimidazo[1,2-a]pyridin-6-yl)-4′-(trifluoromethyl)[1,1′-biphenyl]-4-carboxamide as white solid. Conditions: See react...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
c1ccn2ccnc2c1.C1CC1.c1ccccc1.c1ccccc1
Other
null
null
null
O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1.O=[N+]([O-])c1ccc2nc(C3CC3)cn2c1>>O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-fac5f2b041624d1c8c5de8b4c0b5b93e
O=C(O)c1ccc(-c2ccc(Cl)cn2)cc1.O=[N+]([O-])c1ccc2nc(C3CC3)cn2c1>>O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ccc(-c2ccc(Cl)cn2)cc1
C1(CC1)C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1.ClC=1C=CC(=NC1)C1=CC=C(C=C1)C(=O)O>>ClC=1C=CC(=NC1)C1=CC=C(C(=O)NC=2C=CC=3N(C2)C=C(N3)C3CC3)C=C1
O[C:2](=[O:1])[c:16]1[cH:17][cH:18][c:19](-[c:20]2[cH:21][cH:22][c:23]([Cl:24])[cH:25][n:26]2)[cH:27][cH:28]1.O=[N+:3]([O-])[c:4]1[cH:5][cH:6][c:7]2[n:8][c:9]([CH:10]3[CH2:11][CH2:12]3)[cH:13][n:14]2[cH:15]1>>[O:1]=[C:2]([NH:3][c:4]1[cH:5][cH:6][c:7]2[n:8][c:9]([CH:10]3[CH2:11][CH2:12]3)[cH:13][n:14]2[cH:15]1)[c:16]1[c...
O=C(O)c1ccc(-c2ccc(Cl)cn2)cc1.O=[N+]([O-])c1ccc2nc(C3CC3)cn2c1
O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ccc(-c2ccc(Cl)cn2)cc1
null
null
null
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ccc(-c2ccccn2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[N+;H0;D3:6](-[O-])-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[c:12]:[#7;a:13]:[c:14]:1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
Operations similar to those of Example 1 were conducted using 2-cyclopropyl-6-nitroimidazo[1,2-a]pyridine and 4-(5-chloro-2-pyridyl)benzenecarboxylic acid, to provide 4-(5-chloro-2-pyridyl)-N-(2-cyclopropylimidazo[1,2-a]pyridine-6-yl)benzamide as white solid. Further treating the resulting compound in the manner simila...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
c1ccn2ccnc2c1.C1CC1.c1ccccc1.c1ccncc1
Other
null
null
null
O=C(O)c1ccc(-c2ccc(Cl)cn2)cc1.O=[N+]([O-])c1ccc2nc(C3CC3)cn2c1>>O=C(Nc1ccc2nc(C3CC3)cn2c1)c1ccc(-c2ccc(Cl)cn2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f235ba78a7b243babcbba2117626aae8
Cc1c(N(C)C(=O)C(F)(F)F)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1>>Cc1c(N(C)C(=O)C(F)(F)F)nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cc4)cc3)cn12
FC(C(=O)N(C=1N=C2N(C=C(C=C2)[N+](=O)[O-])C1C)C)(F)F.FC(C1=CC=C(C=C1)C1=CC=C(C=C1)C(=O)O)(F)F>>CC1=C(N=C2N1C=C(C=C2)NC(=O)C2=CC=C(C=C2)C2=CC=C(C=C2)C(F)(F)F)N(C(C(F)(F)F)=O)C
O=[N+:17]([O-])[c:16]1[cH:15][cH:14][c:13]2[n:12][c:3]([N:4]([CH3:5])[C:6](=[O:7])[C:8]([F:9])([F:10])[F:11])[c:2]([CH3:1])[n:37]2[cH:36]1.O[C:18](=[O:19])[c:20]1[cH:21][cH:22][c:23](-[c:24]2[cH:25][cH:26][c:27]([C:28]([F:29])([F:30])[F:31])[cH:32][cH:33]2)[cH:34][cH:35]1>>[CH3:1][c:2]1[c:3]([N:4]([CH3:5])[C:6](=[O:7])...
Cc1c(N(C)C(=O)C(F)(F)F)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1
Cc1c(N(C)C(=O)C(F)(F)F)nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cc4)cc3)cn12
null
null
null
Acylation
OtherReaction
07d1695adb57fcbe166e427114577c880df19df2ee26bdadcbdf979c1785ff55
141f63f004bbbe912fc54e457ad7143d740953538a28293f72b74ca32c03fab9
O=C(Nc1ccc2nccn2c1)c1ccc(-c2ccccc2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[N+;H0;D3:6](-[O-])-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[#7;a:12]:[c:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]1:[c:11]:[#7;a:12]:[c:13]:[c:14]:1)-[c:3](:[c:4]):[c:5]
61.2
[{"value": 61.2, "product": "CC1=C(N=C2N1C=C(C=C2)NC(=O)C2=CC=C(C=C2)C2=CC=C(C=C2)C(F)(F)F)N(C(C(F)(F)F)=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Operations similar to Example 1 were conducted using 2,2,2-trifluoro-N-methyl-N-(3-methyl-6-nitroimidazo[1,2-a]pyridin-2-yl)acetamide (580 mg) and 4′-(trifluoromethyl)[1,1′-biphenyl]-4-carboxylic acid (510 mg), to provide N-{3-methyl-2-[methyl(2,2,2-trifluoroacetyl)amino]imidazo[1,2-a]pyridin-6-yl}-4′(trifluoromethyl)-...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
null
c1ccn2ccnc2c1.c1ccccc1.c1ccccc1
Other
null
null
null
Cc1c(N(C)C(=O)C(F)(F)F)nc2ccc([N+](=O)[O-])cn12.O=C(O)c1ccc(-c2ccc(C(F)(F)F)cc2)cc1>>Cc1c(N(C)C(=O)C(F)(F)F)nc2ccc(NC(=O)c3ccc(-c4ccc(C(F)(F)F)cc4)cc3)cn12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-367f9957fbe3451b925fcad46fbcfe08
CC1(C)OCC(CO)O1.CCCCCCCCCCCCCCCCBr>>CCCCCCCCCCCCCCCCOCC(O)CO
[OH-].[K+].C(CCCCCCCCCCCCCCC)Br.CC1(OCC(O1)CO)C>>C(CCCCCCCCCCCCCCC)OCC(O)CO
CC1(C)[O:17][CH2:18][CH:19]([CH2:21][OH:22])[O:20]1.Br[CH2:16][CH2:15][CH2:14][CH2:13][CH2:12][CH2:11][CH2:10][CH2:9][CH2:8][CH2:7][CH2:6][CH2:5][CH2:4][CH2:3][CH2:2][CH3:1]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][CH2:13][CH2:14][CH2:15][CH2:16][O:17][CH2:18][CH:19]([OH:...
CC1(C)OCC(CO)O1.CCCCCCCCCCCCCCCCBr
CCCCCCCCCCCCCCCCOCC(O)CO
null
null
C1=CC=CC=C1.CCOCC
Heteroatom Alkylation and Arylation
OtherReaction
52d9a9d601c7b22ee50eec30dd99222029787a08b6512bd1185a59a4beaa83df
7c129380d3b6717e6dab4e7b3072bb9c9efc6e13cceeaeae34b29769460ca1a3
null
Br-[CH2;D2;+0:1]-[C:2]-[C:3].C-C1(-C)-[O;H0;D2;+0:4]-[C:5]-[C:6](-[C:7])-[O;H0;D2;+0:8]-1>>[C:3]-[C:2]-[CH2;D2;+0:1]-[O;H0;D2;+0:4]-[C:5]-[C:6](-[C:7])-[OH;D1;+0:8]
77.2
[{"value": 77.2, "product": "C(CCCCCCCCCCCCCCC)OCC(O)CO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
D-Acetone glycerol (4 grams) for synthesis of L-ALLE or L-Acetone glycerol for synthesis of D-ALLE, powdered potassium hydroxide (approximately 10 grams) and hexadecyl bromide (9.3 grams) in benzene (100 ml) were stirred and refluxed for 5 hours, while removing the water formed by azeotropic distillation (compare W. J....
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ether.Ether
Ether.Secondary alcohol
C1COCO1
null
null
HBr
C1=CC=CC=C1.CCOCC
null
null
CC1(C)OCC(CO)O1.CCCCCCCCCCCCCCCCBr>C1=CC=CC=C1.CCOCC>CCCCCCCCCCCCCCCCOCC(O)CO
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d290d528d94d46f3887291aa8600b3e6
O=[N+]([O-])c1ccc(F)cc1>>O=[N+]([O-])c1ccccc1
[N+](=O)([O-])C1=CC=C(C=C1)F.C(=O)(O)COC1=C(C=CC=C1)O.[O-]CCCC.[K+]>>[N+](=O)([O-])C1=CC=CC=C1
F[c:7]1[cH:6][cH:5][c:4]([N+:2](=[O:1])[O-:3])[cH:9][cH:8]1>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][cH:7][cH:8][cH:9]1
O=[N+]([O-])c1ccc(F)cc1
O=[N+]([O-])c1ccccc1
null
null
CC(=O)N(C)C
Functional Group Interconversion
Aromatic dehalogenation
b66818d3926a4463fb8e1c3d4a89e94e47b4d46960d4bdb7bcfbeeec427cfd4e
56de34d4a44cb25d9380269ee5e138b0f24b40a3a0db22c5508049dc775a861f
c1ccccc1
F-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]>>[c:3]:[c:2]:[cH;D2;+0:1]:[c:4]:[c:5]
null
[]
null
null
null
null
4-nitro-fluorobenzene and 2-(carboxymethoxy)phenol were reacted together in DMA in the presence of potassium butoxide for 2 hours at 150° C. to yield 4-(2-carboxymethoxy)-phenoxy)nitrobenzene. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1ccccc1
c1ccccc1
c1ccccc1
Other
CC(=O)N(C)C
null
null
O=[N+]([O-])c1ccc(F)cc1>CC(=O)N(C)C>O=[N+]([O-])c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-bad3801cbdd44d1e820687480b1b160f
O=C(O)COc1ccccc1O.O=[N+]([O-])c1ccc(F)cc1>>O=C(O)COc1ccccc1Oc1ccc([N+](=O)[O-])cc1
[N+](=O)([O-])C1=CC=C(C=C1)F.C(=O)(O)COC1=C(C=CC=C1)O.[O-]CCCC.[K+]>>C(=O)(O)COC1=C(OC2=CC=C(C=C2)[N+](=O)[O-])C=CC=C1
[O:1]=[C:2]([OH:3])[CH2:4][O:5][c:6]1[cH:7][cH:8][cH:9][cH:10][c:11]1[OH:12].F[c:13]1[cH:14][cH:15][c:16]([N+:17](=[O:18])[O-:19])[cH:20][cH:21]1>>[O:1]=[C:2]([OH:3])[CH2:4][O:5][c:6]1[cH:7][cH:8][cH:9][cH:10][c:11]1[O:12][c:13]1[cH:14][cH:15][c:16]([N+:17](=[O:18])[O-:19])[cH:20][cH:21]1
O=C(O)COc1ccccc1O.O=[N+]([O-])c1ccc(F)cc1
O=C(O)COc1ccccc1Oc1ccc([N+](=O)[O-])cc1
null
null
CC(=O)N(C)C
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
e4ea1e38252bc3b9c5ec04486386725e6570ab3860d45e337a1d131319bbf0fc
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1ccc(Oc2ccccc2)cc1
F-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[OH;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[c:8]:[c:7](-[O;H0;D2;+0:6]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9]
null
[]
null
null
null
null
4-nitro-fluorobenzene and 2-(carboxymethoxy)phenol were reacted together in DMA in the presence of potassium butoxide for 2 hours at 150° C. to yield 4-(2-carboxymethoxy-phenoxy)nitrobenzene, intermediate 1. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1
HF
CC(=O)N(C)C
null
null
O=C(O)COc1ccccc1O.O=[N+]([O-])c1ccc(F)cc1>CC(=O)N(C)C>O=C(O)COc1ccccc1Oc1ccc([N+](=O)[O-])cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0e820eadf4754ff9a253078911dc2753
COc1ccc2c(c1)C=CCN2>>COc1ccc2ncccc2c1
COC=1C=C2C=CCNC2=CC1.P(=O)(Cl)(Cl)Cl>>COC=1C=C2C=CC=NC2=CC1
[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]2[c:11]([cH:12]1)[CH:10]=[CH:9][CH2:8][NH:7]2>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]2[n:7][cH:8][cH:9][cH:10][c:11]2[cH:12]1
COc1ccc2c(c1)C=CCN2
COc1ccc2ncccc2c1
null
null
C(C)#N
Miscellaneous
OtherReaction
7ffe3cebf575efbc523acf75ea06ed0a5206dc9a6b0e18ee1d47ba78967e3a74
949c4079d4cfdc9fe16404f504e221120066c0603ac761a9f7931fdd0e4dbc8b
c1ccc2ncccc2c1
[c:1]:[c:2]1:[c:3](:[c:4])-[NH;D2;+0:5]-[CH2;D2;+0:6]-[CH;D2;+0:7]=[CH;D2;+0:8]-1>>[c:1]:[c:2]1:[cH;D2;+0:8]:[cH;D2;+0:7]:[cH;D2;+0:6]:[n;H0;D2;+0:5]:[c:3]:1:[c:4]
97
[{"value": 97.0, "product": "COC=1C=C2C=CC=NC2=CC1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
3-cyano, 4-oxo, 6-methoxy dihydroquinoline was reacted with phosphorus oxychloride in acetonitrile at 85° C. for 5 hr to give 3-cyano, 4-chloro, 6-methoxy quinoline 97% purity by HPLC Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Secondary amine
null
C1=Cc2ccccc2NC1
c1ccc2ncccc2c1
c1ccc2ncccc2c1
null
C(C)#N
null
null
COc1ccc2c(c1)C=CCN2>C(C)#N>COc1ccc2ncccc2c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7e59939bc5984fb29736b4935ff5f651
O=C(O)COc1ccccc1O.O=[N+]([O-])c1ccc(F)cc1>>O=C(O)COc1ccccc1Oc1ccc([N+](=O)[O-])cc1
FC1=CC=C(C=C1)[N+](=O)[O-].OC1=C(OCC(=O)O)C=CC=C1.CC(C)([O-])C.[K+].CC(=O)N(C)C>>[N+](=O)([O-])C1=CC=C(OC2=C(OCC(=O)O)C=CC=C2)C=C1
[O:1]=[C:2]([OH:3])[CH2:4][O:5][c:6]1[cH:7][cH:8][cH:9][cH:10][c:11]1[OH:12].F[c:13]1[cH:14][cH:15][c:16]([N+:17](=[O:18])[O-:19])[cH:20][cH:21]1>>[O:1]=[C:2]([OH:3])[CH2:4][O:5][c:6]1[cH:7][cH:8][cH:9][cH:10][c:11]1[O:12][c:13]1[cH:14][cH:15][c:16]([N+:17](=[O:18])[O-:19])[cH:20][cH:21]1
O=C(O)COc1ccccc1O.O=[N+]([O-])c1ccc(F)cc1
O=C(O)COc1ccccc1Oc1ccc([N+](=O)[O-])cc1
null
null
null
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
e4ea1e38252bc3b9c5ec04486386725e6570ab3860d45e337a1d131319bbf0fc
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1ccc(Oc2ccccc2)cc1
F-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[OH;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[c:8]:[c:7](-[O;H0;D2;+0:6]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9]
null
[]
null
null
null
null
4-(fluoro)nitrobenzene was reacted with 2-(2-hydroxyphenoxy)acetic acid in the presence of potassium t-butoxide/DMA at 150° C. for 2 hrs to give 2-[(2-(4-nitrophenoxy)phenoxy] acetic acid. The product was purified by chromatography. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1
HF
null
null
null
O=C(O)COc1ccccc1O.O=[N+]([O-])c1ccc(F)cc1>>O=C(O)COc1ccccc1Oc1ccc([N+](=O)[O-])cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5e378f173bb444b7aee359cc610c6e24
COc1ccnc(Cl)c1.Nc1ccc(O)cc1>>COc1ccnc(Oc2ccc(N)cc2)c1
NC1=CC=C(C=C1)O.COC1=CC(=NC=C1)Cl.CC(C)(C)[O-].[K+]>>NC1=CC=C(OC2=NC=CC(=C2)OC)C=C1
Cl[c:7]1[n:6][cH:5][cH:4][c:3]([O:2][CH3:1])[cH:16]1.[OH:8][c:9]1[cH:10][cH:11][c:12]([NH2:13])[cH:14][cH:15]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][n:6][c:7]([O:8][c:9]2[cH:10][cH:11][c:12]([NH2:13])[cH:14][cH:15]2)[cH:16]1
COc1ccnc(Cl)c1.Nc1ccc(O)cc1
COc1ccnc(Oc2ccc(N)cc2)c1
null
null
CC(=O)N(C)C
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
99925b30dd2603ae575cba81b58435d015cd6b7267cf347380904f25833af5f2
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1ccc(Oc2ccccn2)cc1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5].[OH;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[c:8]:[c:7](-[O;H0;D2;+0:6]-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5]):[c:9]
null
[]
null
null
null
null
4-Aminophenol was reacted with 4-methoxy-2-chloropyridine in the presence of KOtBu/8-Crown-6/DMA at 150° C. for 5 hrs to give 2-(4-aminophenoxy)-4-methoxypyridine. The product was purified by chromatography. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccncc1
c1ccncc1
c1ccncc1.c1ccccc1
HCl
CC(=O)N(C)C
null
null
COc1ccnc(Cl)c1.Nc1ccc(O)cc1>CC(=O)N(C)C>COc1ccnc(Oc2ccc(N)cc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a3d3340515b549119f073eff5ec74b45
Nc1ccc(C(=O)O)cc1N.O=Cc1ccc(Oc2ccc(F)cc2)cc1>>O=C(O)c1ccc2[nH]c(-c3ccc(Oc4ccccc4)cc3)nc2c1
FC1=CC=C(OC2=CC=C(C=O)C=C2)C=C1.NC=1C=C(C(=O)O)C=CC1N.NC=1C=C(C(=O)N)C=CC1N>>O(C1=CC=CC=C1)C1=CC=C(C=C1)C1=NC2=C(N1)C=CC(=C2)C(=O)O
[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][c:7]([NH2:8])[c:24]([NH2:23])[cH:25]1.O=[CH:9][c:10]1[cH:11][cH:12][c:13]([O:14][c:15]2[cH:16][cH:17][c:18](F)[cH:19][cH:20]2)[cH:21][cH:22]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][c:7]2[nH:8][c:9](-[c:10]3[cH:11][cH:12][c:13]([O:14][c:15]4[cH:16][cH:17][cH:18][cH:19][cH:20]4)[cH:2...
Nc1ccc(C(=O)O)cc1N.O=Cc1ccc(Oc2ccc(F)cc2)cc1
O=C(O)c1ccc2[nH]c(-c3ccc(Oc4ccccc4)cc3)nc2c1
null
null
null
Aromatic Heterocycle Formation
OtherReaction
f4ad6a1d90ab5bd0bba8c0e178876500d65d3160b8ab7cc88185242ee3258127
92b3cf8c078f72830f19960a989555674686a3e49e4dfd835e29457519e1be13
c1ccc(Oc2ccc(-c3nc4ccccc4[nH]3)cc2)cc1
F-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O=[CH;D2;+0:6]-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10]:[c:11].[NH2;D1;+0:12]-[c:13](:[c:14]):[c:15](-[NH2;D1;+0:16]):[c:17]>>[c:9]:[c:8]:[c;H0;D3;+0:7](-[c;H0;D3;+0:6]1:[n;H0;D2;+0:12]:[c:13](:[c:14]):[c:15](:[c:17]):[nH;D2;+0:16]:1):[c:10]:[c:11].[c:3]:[c:2]:[cH;D2;+0:1]:[c:4]:[c...
null
[]
null
null
null
null
This compound was prepared according to the methods described in Example 22 and Scheme 3, substituting 4-phenoxybenzaldehyde for 4-(4-fluoro-phenoxy)-benzaldehyde, and 3,4-diaminobenzoic acid for 3,4-diaminobenzoic acid amide. Conditions: See reaction.notes.procedure_details. Workup: This compound was prepared
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aldehyde.Primary amine.Primary amine
null
c1ccccc1.c1ccccc1
c1ccc2[nH]cnc2c1.c1ccccc1
c1ccc2[nH]cnc2c1.c1ccccc1.c1ccccc1
HF
null
null
null
Nc1ccc(C(=O)O)cc1N.O=Cc1ccc(Oc2ccc(F)cc2)cc1>>O=C(O)c1ccc2[nH]c(-c3ccc(Oc4ccccc4)cc3)nc2c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-cc1638d34b704af28d1bf1ec97a8d690
Nc1ccc(S(N)(=O)=O)cc1N.O=Cc1ccc(Oc2ccc(F)cc2)cc1>>NS(=O)(=O)c1ccc2[nH]c(-c3ccc(Oc4ccccc4)cc3)nc2c1
FC1=CC=C(OC2=CC=C(C=O)C=C2)C=C1.NC=1C=C(C=CC1N)S(=O)(=O)N.NC=1C=C(C(=O)N)C=CC1N>>O(C1=CC=CC=C1)C1=CC=C(C=C1)C1=NC2=C(N1)C=CC(=C2)S(=O)(=O)N
[NH2:1][S:2](=[O:3])(=[O:4])[c:5]1[cH:6][cH:7][c:8]([NH2:9])[c:25]([NH2:24])[cH:26]1.O=[CH:10][c:11]1[cH:12][cH:13][c:14]([O:15][c:16]2[cH:17][cH:18][c:19](F)[cH:20][cH:21]2)[cH:22][cH:23]1>>[NH2:1][S:2](=[O:3])(=[O:4])[c:5]1[cH:6][cH:7][c:8]2[nH:9][c:10](-[c:11]3[cH:12][cH:13][c:14]([O:15][c:16]4[cH:17][cH:18][cH:19][...
Nc1ccc(S(N)(=O)=O)cc1N.O=Cc1ccc(Oc2ccc(F)cc2)cc1
NS(=O)(=O)c1ccc2[nH]c(-c3ccc(Oc4ccccc4)cc3)nc2c1
null
null
null
Aromatic Heterocycle Formation
OtherReaction
f4ad6a1d90ab5bd0bba8c0e178876500d65d3160b8ab7cc88185242ee3258127
92b3cf8c078f72830f19960a989555674686a3e49e4dfd835e29457519e1be13
c1ccc(Oc2ccc(-c3nc4ccccc4[nH]3)cc2)cc1
F-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O=[CH;D2;+0:6]-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10]:[c:11].[NH2;D1;+0:12]-[c:13](:[c:14]):[c:15](-[NH2;D1;+0:16]):[c:17]>>[c:9]:[c:8]:[c;H0;D3;+0:7](-[c;H0;D3;+0:6]1:[n;H0;D2;+0:12]:[c:13](:[c:14]):[c:15](:[c:17]):[nH;D2;+0:16]:1):[c:10]:[c:11].[c:3]:[c:2]:[cH;D2;+0:1]:[c:4]:[c...
null
[]
null
null
null
null
This compound was prepared according to the methods described in Example 22 and Scheme 3, substituting 4-phenoxybenzaldehyde for 4-(4-fluoro-phenoxy)-benzaldehyde, and 3,4-diaminobenzene sulfonamide for 3,4-diaminobenzoic acid amide. Conditions: See reaction.notes.procedure_details. Workup: This compound was prepared
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aldehyde.Primary amine.Primary amine
null
c1ccccc1.c1ccccc1
c1ccc2[nH]cnc2c1.c1ccccc1
c1ccc2[nH]cnc2c1.c1ccccc1.c1ccccc1
HF
null
null
null
Nc1ccc(S(N)(=O)=O)cc1N.O=Cc1ccc(Oc2ccc(F)cc2)cc1>>NS(=O)(=O)c1ccc2[nH]c(-c3ccc(Oc4ccccc4)cc3)nc2c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5acdadaf666d404ca4234f7ce496ba9b
Nc1ccc(C=O)cc1.O=S(=O)(Cl)c1ccc(Cl)c(Cl)c1>>O=Cc1ccc(NS(=O)(=O)c2ccc(Cl)c(Cl)c2)cc1
NC1=CC=C(C=O)C=C1.N1=CC=CC=C1.ClC=1C=C(C=CC1Cl)S(=O)(=O)Cl.[N+](=O)([O-])C=1C=C(C=CC1)C1=NC2=C(N1)C=CC(=C2)C(=O)N>>ClC=1C=C(C=CC1Cl)S(=O)(=O)NC1=CC=C(C=C1)C=O
[O:1]=[CH:2][c:3]1[cH:4][cH:5][c:6]([NH2:7])[cH:19][cH:20]1.Cl[S:8](=[O:9])(=[O:10])[c:11]1[cH:12][cH:13][c:14]([Cl:15])[c:16]([Cl:17])[cH:18]1>>[O:1]=[CH:2][c:3]1[cH:4][cH:5][c:6]([NH:7][S:8](=[O:9])(=[O:10])[c:11]2[cH:12][cH:13][c:14]([Cl:15])[c:16]([Cl:17])[cH:18]2)[cH:19][cH:20]1
Nc1ccc(C=O)cc1.O=S(=O)(Cl)c1ccc(Cl)c(Cl)c1
O=Cc1ccc(NS(=O)(=O)c2ccc(Cl)c(Cl)c2)cc1
null
null
C(Cl)Cl
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=S(=O)(Nc1ccccc1)c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[NH2;D1;+0:7]-[c:8](:[c:9]):[c:10]>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[NH;D2;+0:7]-[c:8](:[c:9]):[c:10])-[c:4](:[c:5]):[c:6]
72
[{"value": 72.0, "product": "ClC=1C=C(C=CC1Cl)S(=O)(=O)NC1=CC=C(C=C1)C=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
16
HOUR
2-(3-Nitro-phenyl)-1H-benzoimidazole-5-carboxylic acid amide. To a flask containing crude 4-amino-benzaldehyde (100 mg, 0.82 mmol), pyridine (0.15 mL, 1.87 mmol) and CH2Cl2 (4 mL), was added 3,4-dichlorobenzenesulfonyl chloride (184 mg, 0.75 mmol). The mixture was stirred for 16 h at room temperature, and was then cool...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccccc1.c1ccccc1
HCl
C(Cl)Cl
null
16
Nc1ccc(C=O)cc1.O=S(=O)(Cl)c1ccc(Cl)c(Cl)c1>C(Cl)Cl>O=Cc1ccc(NS(=O)(=O)c2ccc(Cl)c(Cl)c2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1191f8a6159b4c1689edac52db4be715
COc1ccc([N+](=O)[O-])c(N)n1.Nc1nc(Br)ccc1[N+](=O)[O-]>>Br.Nc1nc(O)ccc1[N+](=O)[O-]
BrC1=CC=C(C(=N1)N)[N+](=O)[O-].COC1=CC=C(C(=N1)N)[N+](=O)[O-]>>Br.NC1=C(C=CC(=N1)O)[N+](=O)[O-]
C[O:6][c:5]1[n:4][c:3]([NH2:2])[c:9]([N+:10](=[O:11])[O-:12])[cH:8][cH:7]1.Nc1nc([Br:1])ccc1[N+](=O)[O-]>>[BrH:1].[NH2:2][c:3]1[n:4][c:5]([OH:6])[cH:7][cH:8][c:9]1[N+:10](=[O:11])[O-:12]
COc1ccc([N+](=O)[O-])c(N)n1.Nc1nc(Br)ccc1[N+](=O)[O-]
Br.Nc1nc(O)ccc1[N+](=O)[O-]
null
null
Br.C(C)(=O)O
Miscellaneous
OtherReaction
fd244eb0624fa384b510733d5e039f55f706479d2f18b9df581e8f92d9bb1fa0
3121ad2041919c6e76386d177bdfc4d5d056f74749761519904b3ec281c20584
c1ccncc1
C-[O;H0;D2;+0:1]-[c:2](:[c:3]):[#7;a:4]:[c:5].N-c1:n:c(-[Br;H0;D1;+0:6]):c:c:c:1-[N+](=O)-[O-]>>[BrH;D0;+0:6].[OH;D1;+0:1]-[c:2](:[c:3]):[#7;a:4]:[c:5]
95
[{"value": 95.0, "product": "Br.NC1=C(C=CC(=N1)O)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}]
60
CELSIUS
null
null
6-Bromo-3-nitro-pyridin-2-ylamine. To a glass pressure vessel containing 6-methoxy-3-nitro-pyridin-2-ylamine (5.0 g, 29.5 mmol) was added 30% hydrogen bromide/acetic acid (60 mL). The vessel was sealed, and the contents were heated to 60° C. for 24 h. The reaction mixture was cooled, and the solvent was removed in vacu...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ether.Nitro group.Primary amine
Aromatic alcohol
c1ccncc1
null
c1ccncc1
HO-
Br.C(C)(=O)O
60
null
COc1ccc([N+](=O)[O-])c(N)n1.Nc1nc(Br)ccc1[N+](=O)[O-]>Br.C(C)(=O)O>Br.Nc1nc(O)ccc1[N+](=O)[O-]
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2c6e0c3e1bcd45b8adc124b33ba845ca
N#Cc1ccc([N+](=O)[O-])c(N)n1>>N#Cc1ccc(N)c(N)n1
ClC=1C=C(OC2=CC=C(C=C2)C=2NC=3C(=NC(=CC3)C(=O)N)N2)C=CC1Cl.NC1=C(C=CC(=N1)C#N)[N+](=O)[O-]>>NC=1C=CC(=NC1N)C#N
O=[N+:7]([O-])[c:6]1[cH:5][cH:4][c:3]([C:2]#[N:1])[n:10][c:8]1[NH2:9]>>[N:1]#[C:2][c:3]1[cH:4][cH:5][c:6]([NH2:7])[c:8]([NH2:9])[n:10]1
N#Cc1ccc([N+](=O)[O-])c(N)n1
N#Cc1ccc(N)c(N)n1
null
[Pd]
C(C)O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccncc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4](-[N;D1;H2:5]):[#7;a:6]:[c:7]>>[N;D1;H2:5]-[c:4](:[#7;a:6]:[c:7]):[c:2](-[NH2;D1;+0:1]):[c:3]
null
[]
null
null
3
HOUR
2-[4-(3,4-Dichloro-phenoxy)-phenyl]-1H-imidazo[4,5-b]pyridine-5-carboxylic acid amide. A flask containing 6-amino-5-nitro-pyridine-2-carbonitrile (67 mg, 0.40 mmol), 10% palladium on carbon (catalytic) and ethanol (2.0 mL) was put under an atmosphere of H2 using a balloon. The mixture was stirred at room temperature fo...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccncc1
Other
[Pd].C(C)O
null
3
N#Cc1ccc([N+](=O)[O-])c(N)n1>[Pd].C(C)O>N#Cc1ccc(N)c(N)n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3ae7c85dcc914422a8b0b8fde6dc8647
N#Cc1ccc2[nH]c(-c3ccc(Oc4ccc(Cl)c(Cl)c4)cc3)nc2n1.O=Cc1ccc(Oc2ccc(Cl)c(Cl)c2)cc1>>NC(=O)c1ccc2[nH]c(-c3ccc(Oc4ccc(Cl)c(Cl)c4)cc3)nc2n1
NC=1C=CC(=NC1N)C#N.ClC=1C=C(OC2=CC=C(C=O)C=C2)C=CC1Cl.CN(C(C)=O)C.ClC=1C=C(OC2=CC=C(C=C2)C=2NC=3C(=NC(=CC3)C#N)N2)C=CC1Cl>>ClC=1C=C(OC2=CC=C(C=C2)C=2NC=3C(=NC(=CC3)C(=O)N)N2)C=CC1Cl
[N:1]#[C:2][c:4]1[cH:5][cH:6][c:7]2[nH:8][c:9](-[c:10]3[cH:11][cH:12][c:13]([O:14][c:15]4[cH:16][cH:17][c:18]([Cl:19])[c:20]([Cl:21])[cH:22]4)[cH:23][cH:24]3)[n:25][c:26]2[n:27]1.Clc1ccc(Oc2ccc(C=[O:3])cc2)cc1Cl>>[NH2:1][C:2](=[O:3])[c:4]1[cH:5][cH:6][c:7]2[nH:8][c:9](-[c:10]3[cH:11][cH:12][c:13]([O:14][c:15]4[cH:16][c...
N#Cc1ccc2[nH]c(-c3ccc(Oc4ccc(Cl)c(Cl)c4)cc3)nc2n1.O=Cc1ccc(Oc2ccc(Cl)c(Cl)c2)cc1
NC(=O)c1ccc2[nH]c(-c3ccc(Oc4ccc(Cl)c(Cl)c4)cc3)nc2n1
null
null
O.[OH-].[Na+]
Miscellaneous
OtherReaction
38473d65287697bacdad8a7b056914277e32da57df3acbc08d05ff2609af29fd
e976a573cc0fcfe5bcdced9e9aff2126e2e85772ccca42fd78bff9c131b70e83
c1ccc(Oc2ccc(-c3nc4ncccc4[nH]3)cc2)cc1
Cl-c1:c:c:c(-O-c2:c:c:c(-C=[O;H0;D1;+0:1]):c:c:2):c:c:1-Cl.[#7;a:2]:[c:3](:[#7;a:4]:[c:5](-[C;H0;D2;+0:6]#[N;H0;D1;+0:7]):[c:8]):[c:9]:[#7;a:10]>>[#7;a:2]:[c:3](:[#7;a:4]:[c:5](-[C;H0;D3;+0:6](-[NH2;D1;+0:7])=[O;H0;D1;+0:1]):[c:8]):[c:9]:[#7;a:10]
94.6
[{"value": 94.0, "product": "ClC=1C=C(OC2=CC=C(C=C2)C=2NC=3C(=NC(=CC3)C(=O)N)N2)C=CC1Cl", "details": "PERCENTYIELD", "is_desired": false}, {"value": 94.6, "product": "ClC=1C=C(OC2=CC=C(C=C2)C=2NC=3C(=NC(=CC3)C(=O)N)N2)C=CC1Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
120
CELSIUS
24
HOUR
2-[4-(3,4-Dichloro-phenoxy)-phenyl]-1H-imidazo[4,5-b]pyridine-5-carboxylic acid amide. A flask containing 6-amino-5-nitro-pyridine-2-carbonitrile (67 mg, 0.40 mmol), 10% palladium on carbon (catalytic) and ethanol (2.0 mL) was put under an atmosphere of H2 using a balloon. The mixture was stirred at room temperature fo...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide.Aldehyde.Ether.Nitrile
Primary amide
c1ccccc1.c1ccccc1
null
c1cnc2nc[nH]c2c1.c1ccccc1.c1ccccc1
HCl
O.[OH-].[Na+]
120
24
N#Cc1ccc2[nH]c(-c3ccc(Oc4ccc(Cl)c(Cl)c4)cc3)nc2n1.O=Cc1ccc(Oc2ccc(Cl)c(Cl)c2)cc1>O.[OH-].[Na+]>NC(=O)c1ccc2[nH]c(-c3ccc(Oc4ccc(Cl)c(Cl)c4)cc3)nc2n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-bc0a2177da05457c832f6830b0535dce
NC(=O)c1ccc(N)c(N)c1.Nc1ccc(S(N)(=O)=O)cc1N.O=Cc1ccc(Oc2ccc(F)cc2)cc1>>NS(=O)(=O)c1ccc2[nH]c(-c3ccc(Oc4ccc5ccccc5c4)cc3)nc2c1
FC1=CC=C(OC2=CC=C(C=O)C=C2)C=C1.NC=1C=C(C=CC1N)S(=O)(=O)N.NC=1C=C(C(=O)N)C=CC1N>>C1=C(C=CC2=CC=CC=C12)OC1=CC=C(C=C1)C1=NC2=C(N1)C=CC(=C2)S(=O)(=O)N
Nc1c[c:21]([C:20](N)=O)[cH:22][cH:23]c1N.[NH2:1][S:2](=[O:3])(=[O:4])[c:5]1[cH:6][cH:7][c:8]([NH2:9])[c:29]([NH2:28])[cH:30]1.O=[CH:10][c:11]1[cH:12][cH:13][c:14]([O:15][c:16]2[cH:17][cH:18][c:19](F)[cH:24][cH:25]2)[cH:26][cH:27]1>>[NH2:1][S:2](=[O:3])(=[O:4])[c:5]1[cH:6][cH:7][c:8]2[nH:9][c:10](-[c:11]3[cH:12][cH:13][...
NC(=O)c1ccc(N)c(N)c1.Nc1ccc(S(N)(=O)=O)cc1N.O=Cc1ccc(Oc2ccc(F)cc2)cc1
NS(=O)(=O)c1ccc2[nH]c(-c3ccc(Oc4ccc5ccccc5c4)cc3)nc2c1
null
null
null
Aromatic Heterocycle Formation
OtherReaction
e5075026627231d073a25a05046f833469f27df49a9f3ef757543e8ac4c05b02
40f1e50ea82c16740a65162deb303e490e5736faef43c3e243b1134bf8d54295
c1ccc2cc(Oc3ccc(-c4nc5ccccc5[nH]4)cc3)ccc2c1
F-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[c:5]:[cH;D2;+0:6]:1.O=[CH;D2;+0:7]-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12].N-[C;H0;D3;+0:13](=O)-[c;H0;D3;+0:14]1:[c:15]:[cH;D2;+0:16]:c(-N):c(-N):c:1.[NH2;D1;+0:17]-[c:18](:[c:19]):[c:20](-[NH2;D1;+0:21]):[c:22]>>[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1]2:[cH;D2;+0:13]:[cH;D2;+0:14]:[c...
null
[]
null
null
null
null
This compound was prepared according to the methods described in Example 22 and Scheme 3, substituting 4-(naphthalen-2-yloxy)-benzaldehyde for 4-(4-fluoro-phenoxy)-benzaldehyde, and 3,4-diamino-benzenesulfonamide for 3,4-diaminobenzamide. Conditions: See reaction.notes.procedure_details. Workup: This compound was prepa...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aldehyde.Primary amide.Primary amine.Primary amine.Primary amine.Primary amine
null
c1ccccc1.c1ccccc1.c1ccccc1
c1ccc2[nH]cnc2c1.c1ccc2ccccc2c1
c1ccc2[nH]cnc2c1.c1ccccc1.c1ccc2ccccc2c1
HF
null
null
null
NC(=O)c1ccc(N)c(N)c1.Nc1ccc(S(N)(=O)=O)cc1N.O=Cc1ccc(Oc2ccc(F)cc2)cc1>>NS(=O)(=O)c1ccc2[nH]c(-c3ccc(Oc4ccc5ccccc5c4)cc3)nc2c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b69f37ad842d46b3aeb6be2812aebbb8
O=C(OCc1ccccc1)N1CC=CCC1.O=C(OO)c1cccc(Cl)c1>>O=C(OCc1ccccc1)N1CCC2OC2C1
N1(CCC=CC1)C(=O)OCC1=CC=CC=C1.ClC=1C=C(C(=O)OO)C=CC1.CCCCCC.C(C)(=O)OCC>>C12CN(CCC2O1)C(=O)OCC1=CC=CC=C1
[O:1]=[C:2]([O:3][CH2:4][c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1)[N:11]1[CH2:12][CH2:13][CH:14]=[CH:16][CH2:17]1.O=C(O[OH:15])c1cccc(Cl)c1>>[O:1]=[C:2]([O:3][CH2:4][c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1)[N:11]1[CH2:12][CH2:13][CH:14]2[O:15][CH:16]2[CH2:17]1
O=C(OCc1ccccc1)N1CC=CCC1.O=C(OO)c1cccc(Cl)c1
O=C(OCc1ccccc1)N1CCC2OC2C1
null
null
ClCCl
Heteroatom Alkylation and Arylation
OtherReaction
3b45a1ce172e737dc524e1c5169806f7804897994baa710a8d301697bf4df36f
c40ffbbc3249442e5ee39aaa69a55be7ac2fa45f48637395e415c565c1288454
O=C(OCc1ccccc1)N1CCC2OC2C1
Cl-c1:c:c:c:c(-C(=O)-O-[OH;D1;+0:1]):c:1.[#8:2]-[C:3](=[O;D1;H0:4])-[#7:5]1-[C:6]-[C:7]-[CH;D2;+0:8]=[CH;D2;+0:9]-[C:10]-1>>[#8:2]-[C:3](=[O;D1;H0:4])-[#7:5]1-[C:6]-[C:7]-[CH;D3;+0:8]2-[O;H0;D2;+0:1]-[CH;D3;+0:9]-2-[C:10]-1
null
[]
null
null
null
null
A stirred solution of benzyl 3,6-dihydropyridine-1(2H)-carboxylate (20.0 g, 92.0 mmol) in dichloromethane (280 ml) was cooled to 0° C. A solution of m-chloroperoxybenzoic acid (22.5 g, approx. 130 mmol) in dichloromethane (560 ml) was added drop-wise and the resulting colourless reaction mixture warmed to room temperat...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Peroxide
Ether
C1=CC[NH]CC1.c1ccccc1
C1CC2OC2C[NH]1
c1ccccc1.C1CC2OC2C[NH]1
HCl
ClCCl
null
null
O=C(OCc1ccccc1)N1CC=CCC1.O=C(OO)c1cccc(Cl)c1>ClCCl>O=C(OCc1ccccc1)N1CCC2OC2C1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7baff472628c4fd88598f675370fa9fd
Cc1cccc(O)c1C.O=C(OCc1ccccc1)N1CCC2OC2C1>>Cc1cccc(O[C@@H]2CCN(C(=O)OCc3ccccc3)C[C@H]2O)c1C
C12CN(CCC2O1)C(=O)OCC1=CC=CC=C1.CC1=C(C=CC=C1C)O.[OH-].[Na+].[OH-].[Na+]>>C(C1=CC=CC=C1)OC(=O)N1C[C@H]([C@@H](CC1)OC1=C(C(=CC=C1)C)C)O
[CH3:1][c:2]1[cH:3][cH:4][cH:5][c:6]([OH:7])[c:25]1[CH3:26].[CH:8]12[CH2:9][CH2:10][N:11]([C:12](=[O:13])[O:14][CH2:15][c:16]3[cH:17][cH:18][cH:19][cH:20][cH:21]3)[CH2:22][CH:23]1[O:24]2>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][c:6]([O:7][C@@H:8]2[CH2:9][CH2:10][N:11]([C:12](=[O:13])[O:14][CH2:15][c:16]3[cH:17][cH:18][cH:19][c...
Cc1cccc(O)c1C.O=C(OCc1ccccc1)N1CCC2OC2C1
Cc1cccc(O[C@@H]2CCN(C(=O)OCc3ccccc3)C[C@H]2O)c1C
null
null
C(C)#N.[Cl-].[Na+].O.O
Heteroatom Alkylation and Arylation
OtherReaction
bb8a59912df33eb4894501658fa75b47f44d0cef1868e510b68ee039cf0ab21b
d65f28c52f0777a08a008cfdcfc030aaa24bdbbd95c8114c9f5ad2abd4641bd1
O=C(OCc1ccccc1)N1CCC(Oc2ccccc2)CC1
[#8:1]-[C:2](=[O;D1;H0:3])-[#7:4]1-[C:5]-[C:6]-[CH;D3;+0:7]2-[O;H0;D2;+0:8]-[CH;D3;+0:9]-2-[C:10]-1.[OH;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[#8:1]-[C:2](=[O;D1;H0:3])-[#7:4]1-[C:5]-[C:6]-[C@@H;D3;+0:7](-[O;H0;D2;+0:11]-[c:12](:[c:13]):[c:14])-[C@H;D3;+0:9](-[OH;D1;+0:8])-[C:10]-1
51.4
[{"value": 50.0, "product": "C(C1=CC=CC=C1)OC(=O)N1C[C@H]([C@@H](CC1)OC1=C(C(=CC=C1)C)C)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 51.4, "product": "C(C1=CC=CC=C1)OC(=O)N1C[C@H]([C@@H](CC1)OC1=C(C(=CC=C1)C)C)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Benzyl 7-oxa-3-azabicyclo[4.1.0]heptane-3-carboxylate (21.0 g, 92.0 mmol) was added to a stirred solution of 2,3-dimethylphenol (23.0 g, 188 mmol) and aqueous sodium hydroxide (100 ml, 2N, 200 mmol) in acetonitrile (400 ml). The reaction mixture was heated at reflux for 14 h. On cooling to room temperature, the reactio...
10.6084/m9.figshare.5104873.v1
null
Ether.Aromatic alcohol
Ether.Secondary alcohol
C1CC2OC2C[NH]1
C1CC[NH]CC1
c1ccccc1.C1CC[NH]CC1.c1ccccc1
null
C(C)#N.[Cl-].[Na+].O.O
null
null
Cc1cccc(O)c1C.O=C(OCc1ccccc1)N1CCC2OC2C1>C(C)#N.[Cl-].[Na+].O.O>Cc1cccc(O[C@@H]2CCN(C(=O)OCc3ccccc3)C[C@H]2O)c1C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-96b3a4f7aed34438ba947e698b0b69ad
Cc1cccc(O[C@@H]2CCN(C(=O)OCc3ccccc3)C[C@H]2O)c1C>>Cc1cccc(O[C@@H]2CCNC[C@H]2O)c1C
C(C)OCC.CC1=C(O[C@H]2[C@@H](CN(CC2)C(=O)OCC2=CC=CC=C2)O)C=CC=C1C.[H][H]>>CC1=C(O[C@H]2[C@@H](CNCC2)O)C=CC=C1C
O=C(OCc1ccccc1)[N:11]1[CH2:10][CH2:9][C@@H:8]([O:7][c:6]2[cH:5][cH:4][cH:3][c:2]([CH3:1])[c:15]2[CH3:16])[C@H:13]([OH:14])[CH2:12]1>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][c:6]([O:7][C@@H:8]2[CH2:9][CH2:10][NH:11][CH2:12][C@H:13]2[OH:14])[c:15]1[CH3:16]
Cc1cccc(O[C@@H]2CCN(C(=O)OCc3ccccc3)C[C@H]2O)c1C
Cc1cccc(O[C@@H]2CCNC[C@H]2O)c1C
null
[Pd]
CO
Reduction
Hydrogenolysis of tertiary amines
ce0208fabe82d1244d7db7b6f7627b1b39a8cf3492e02720426849e93718e81c
20c36f41eeb07c3ba4437b51ba72e8ff3c22d0b27e7197b0e9af3127f331149f
c1ccc(OC2CCNCC2)cc1
O=C(-O-C-c1:c:c:c:c:c:1)-[N;H0;D3;+0:1](-[C:2]-[C:3])-[C:4]-[C:5]>>[C:5]-[C:4]-[NH;D2;+0:1]-[C:2]-[C:3]
50
[{"value": 50.0, "product": "CC1=C(O[C@H]2[C@@H](CNCC2)O)C=CC=C1C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 46.6, "product": "CC1=C(O[C@H]2[C@@H](CNCC2)O)C=CC=C1C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of trans-benzyl 4-(2,3-dimethylphenoxy)-3-hydroxypiperidine-1-carboxylate (3.5 g, 9.8 mmol) in methanol (50 ml) was added to 5% palladium on charcoal (350 mg) under an atmosphere of nitrogen. The vessel was placed under an atmosphere of hydrogen and stirred vigorously until hydrogen uptake ceased. The result...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether
Secondary amine
c1ccccc1.C1CC[NH]CC1
C1CCNCC1
c1ccccc1.C1CCNCC1
HO-
[Pd].CO
null
null
Cc1cccc(O[C@@H]2CCN(C(=O)OCc3ccccc3)C[C@H]2O)c1C>[Pd].CO>Cc1cccc(O[C@@H]2CCNC[C@H]2O)c1C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-396c21b53fe14c60a2218777356825ad
Cc1cccc(O[C@@H]2CCN(C(=O)OCc3ccccc3)C[C@H]2O)c1C>>Cc1cccc(OC2CCN(C(=O)OCc3ccccc3)CC2=O)c1C
C(C)N(CC)CC.CS(=O)C.C(C(=O)Cl)(=O)Cl.C(C1=CC=CC=C1)OC(=O)N1C[C@H]([C@@H](CC1)OC1=C(C(=CC=C1)C)C)O>>CC1=C(OC2C(CN(CC2)C(=O)OCC2=CC=CC=C2)=O)C=CC=C1C
[CH3:1][c:2]1[cH:3][cH:4][cH:5][c:6]([O:7][C@@H:8]2[CH2:9][CH2:10][N:11]([C:12](=[O:13])[O:14][CH2:15][c:16]3[cH:17][cH:18][cH:19][cH:20][cH:21]3)[CH2:22][C@H:23]2[OH:24])[c:25]1[CH3:26]>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][c:6]([O:7][CH:8]2[CH2:9][CH2:10][N:11]([C:12](=[O:13])[O:14][CH2:15][c:16]3[cH:17][cH:18][cH:19][cH:...
Cc1cccc(O[C@@H]2CCN(C(=O)OCc3ccccc3)C[C@H]2O)c1C
Cc1cccc(OC2CCN(C(=O)OCc3ccccc3)CC2=O)c1C
null
null
ClCCl.O
Oxidation
Oxidation or Dehydrogenation of Alcohols to Aldehydes and Ketones
eb1454704a72f81f212192eafcb78e0711de77dd6074b9d7e49d38205debb755
767cfd93f5821ebb9e1e72addd9cb404b20b0c821d246ae6b87a5776b74a455b
O=C1CN(C(=O)OCc2ccccc2)CCC1Oc1ccccc1
[#8:1]-[C:2](=[O;D1;H0:3])-[#7:4]1-[C:5]-[C:6]-[C@@H;D3;+0:7](-[#8:8]-[c:9])-[C@H;D3;+0:10](-[OH;D1;+0:11])-[C:12]-1>>[#8:1]-[C:2](=[O;D1;H0:3])-[#7:4]1-[C:5]-[C:6]-[CH;D3;+0:7](-[#8:8]-[c:9])-[C;H0;D3;+0:10](=[O;H0;D1;+0:11])-[C:12]-1
99.2
[{"value": 99.0, "product": "CC1=C(OC2C(CN(CC2)C(=O)OCC2=CC=CC=C2)=O)C=CC=C1C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 99.2, "product": "CC1=C(OC2C(CN(CC2)C(=O)OCC2=CC=CC=C2)=O)C=CC=C1C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-60
CELSIUS
10
MINUTE
A solution of oxalyl chloride (3.5 ml, 40 mmol, 1.1 eq.) in dichloromethane (350 ml) was cooled to −60° C. (internal temp.) and treated drop-wise with dimethyl sulfoxide (5.18 ml, 73.0 mmol, 2 eq.). On completion of addition the reaction mixture was stirred at −60° C. for 5 min. before drop-wise addition of a solution ...
10.6084/m9.figshare.5104873.v1
null
Secondary alcohol
Ketone
C1CC[NH]CC1
C1CC[NH]CC1
c1ccccc1.C1CC[NH]CC1.c1ccccc1
null
ClCCl.O
-60
0.166667
Cc1cccc(O[C@@H]2CCN(C(=O)OCc3ccccc3)C[C@H]2O)c1C>ClCCl.O>Cc1cccc(OC2CCN(C(=O)OCc3ccccc3)CC2=O)c1C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-973ad7ec4b5643c7b0572e224911b650
Cc1cccc(OC2CCN(C(=O)OCc3ccccc3)CC2=O)c1C>>Cc1cccc(O[C@H]2CCN(C(=O)OCc3ccccc3)C[C@H]2O)c1C
CC1=C(OC2C(CN(CC2)C(=O)OCC2=CC=CC=C2)=O)C=CC=C1C.CCC([BH-](C(CC)C)C(CC)C)C.[K+]>>CC1=C(O[C@@H]2[C@@H](CN(CC2)C(=O)OCC2=CC=CC=C2)O)C=CC=C1C
[CH3:1][c:2]1[cH:3][cH:4][cH:5][c:6]([O:7][CH:8]2[CH2:9][CH2:10][N:11]([C:12](=[O:13])[O:14][CH2:15][c:16]3[cH:17][cH:18][cH:19][cH:20][cH:21]3)[CH2:22][C:23]2=[O:24])[c:25]1[CH3:26]>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][c:6]([O:7][C@H:8]2[CH2:9][CH2:10][N:11]([C:12](=[O:13])[O:14][CH2:15][c:16]3[cH:17][cH:18][cH:19][cH:20]...
Cc1cccc(OC2CCN(C(=O)OCc3ccccc3)CC2=O)c1C
Cc1cccc(O[C@H]2CCN(C(=O)OCc3ccccc3)C[C@H]2O)c1C
null
null
O1CCCC1
Reduction
Reduction of ketone to secondary alcohol
c5c426998ef8289eab8bc31f16e2cce4176e0d9dc4e6b9619a0e750a805cc770
1bd3cd74b454139c0a0068ac0135836499926b274bff569df163210c6c944a89
O=C(OCc1ccccc1)N1CCC(Oc2ccccc2)CC1
[#8:1]-[C:2](=[O;D1;H0:3])-[#7:4]1-[C:5]-[C:6]-[CH;D3;+0:7](-[#8:8]-[c:9])-[C;H0;D3;+0:10](=[O;H0;D1;+0:11])-[C:12]-1>>[#8:1]-[C:2](=[O;D1;H0:3])-[#7:4]1-[C:5]-[C:6]-[C@H;D3;+0:7](-[#8:8]-[c:9])-[C@H;D3;+0:10](-[OH;D1;+0:11])-[C:12]-1
50.3
[{"value": 50.0, "product": "CC1=C(O[C@@H]2[C@@H](CN(CC2)C(=O)OCC2=CC=CC=C2)O)C=CC=C1C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 50.3, "product": "CC1=C(O[C@@H]2[C@@H](CN(CC2)C(=O)OCC2=CC=CC=C2)O)C=CC=C1C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
18
HOUR
A solution of benzyl 4-(2,3-dimethylphenoxy)-3-oxopiperidine-1-carboxylate (10.0 g, 28.0 mmol) in tetrahydrofuran (60 ml) was treated at room temperature with K-selectride (10.0M in tetrahydrofuran, 56 ml, 56.0 mmol). On completion of addition the mixture was stirred at room temperature for 18 h. The mixture was concen...
10.6084/m9.figshare.5104873.v1
null
Ketone
Secondary alcohol
C1CC[NH]CC1
C1CC[NH]CC1
c1ccccc1.C1CC[NH]CC1.c1ccccc1
null
O1CCCC1
null
18
Cc1cccc(OC2CCN(C(=O)OCc3ccccc3)CC2=O)c1C>O1CCCC1>Cc1cccc(O[C@H]2CCN(C(=O)OCc3ccccc3)C[C@H]2O)c1C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c573509549f044fb815c0bbb196f3969
Cc1cccc(O[C@H]2CCN(C(=O)OCc3ccccc3)C[C@H]2O)c1C>>Cc1cccc(O[C@H]2CCNC[C@H]2O)c1C
C(C)OCC.CC1=C(O[C@@H]2[C@@H](CN(CC2)C(=O)OCC2=CC=CC=C2)O)C=CC=C1C.[H][H]>>CC1=C(O[C@@H]2[C@@H](CNCC2)O)C=CC=C1C
O=C(OCc1ccccc1)[N:11]1[CH2:10][CH2:9][C@H:8]([O:7][c:6]2[cH:5][cH:4][cH:3][c:2]([CH3:1])[c:15]2[CH3:16])[C@H:13]([OH:14])[CH2:12]1>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][c:6]([O:7][C@H:8]2[CH2:9][CH2:10][NH:11][CH2:12][C@H:13]2[OH:14])[c:15]1[CH3:16]
Cc1cccc(O[C@H]2CCN(C(=O)OCc3ccccc3)C[C@H]2O)c1C
Cc1cccc(O[C@H]2CCNC[C@H]2O)c1C
null
[Pd]
CO
Reduction
Hydrogenolysis of tertiary amines
ce0208fabe82d1244d7db7b6f7627b1b39a8cf3492e02720426849e93718e81c
20c36f41eeb07c3ba4437b51ba72e8ff3c22d0b27e7197b0e9af3127f331149f
c1ccc(OC2CCNCC2)cc1
O=C(-O-C-c1:c:c:c:c:c:1)-[N;H0;D3;+0:1](-[C:2]-[C:3])-[C:4]-[C:5]>>[C:5]-[C:4]-[NH;D2;+0:1]-[C:2]-[C:3]
67.8
[{"value": 67.0, "product": "CC1=C(O[C@@H]2[C@@H](CNCC2)O)C=CC=C1C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 67.8, "product": "CC1=C(O[C@@H]2[C@@H](CNCC2)O)C=CC=C1C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of cis-benzyl 4-(2,3-dimethylphenoxy)-3-hydroxypiperidine-1-carboxylate (5.0 g, 14.0 mmol) in methanol (60 ml) was added to 5% palladium on charcoal (500 mg) under an atmosphere of nitrogen. The vessel was placed under an atmosphere of hydrogen and stirred vigorously until hydrogen uptake ceased. The resulti...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether
Secondary amine
c1ccccc1.C1CC[NH]CC1
C1CCNCC1
c1ccccc1.C1CCNCC1
HO-
[Pd].CO
null
null
Cc1cccc(O[C@H]2CCN(C(=O)OCc3ccccc3)C[C@H]2O)c1C>[Pd].CO>Cc1cccc(O[C@H]2CCNC[C@H]2O)c1C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f9c4481bb48a47a886927688fde45bbe
Cc1cccc([C@@H]2CCNC[C@@H]2O)c1C.Cc1cccc([C@H]2CCNC[C@H]2O)c1C>>Cc1cccc(OC2CCNCC2O)c1C
CC1=C(C=CC=C1C)[C@H]1[C@@H](CNCC1)O.CC1=C(C=CC=C1C)[C@@H]1[C@@H](CNCC1)O.CC1=C(C=CC=C1C)[C@H]1[C@H](CNCC1)O.CC1=C(C=CC=C1C)[C@@H]1[C@H](CNCC1)O>>CC1=C(OC2C(CNCC2)O)C=CC=C1C
[C@@H]1([c:6]2[cH:5][cH:4][cH:3][c:2]([CH3:1])[c:15]2[CH3:16])[CH2:9][CH2:10][NH:11][CH2:12][C@@H:13]1[OH:14].Cc1cccc([C@H]2CCNC[C@H:8]2[OH:7])c1C>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][c:6]([O:7][CH:8]2[CH2:9][CH2:10][NH:11][CH2:12][CH:13]2[OH:14])[c:15]1[CH3:16]
Cc1cccc([C@@H]2CCNC[C@@H]2O)c1C.Cc1cccc([C@H]2CCNC[C@H]2O)c1C
Cc1cccc(OC2CCNCC2O)c1C
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
1b25e45d396e9c0ced225d820a8ceaf13be14b7e03cd644e1c97c0031412c26d
3c33ee7e8620215cdaf497cf199c7a1ad4a7c326860e108d12ae7b3ecae18255
c1ccc(OC2CCNCC2)cc1
null
null
[]
null
null
null
null
Retention times were as follows: (3S,4R)-4-(2,3-dimethylphenyl)-3-hydroxypiperidine, 14.5 minutes; (3R,4S)-4-(2,3-dimethylphenyl)-3-hydroxypiperidine, 16.5 minutes; (3R,4R)-4-(2,3-dimethylphenyl)-3-hydroxypiperidine, 15 minutes; and nM (3S,4S)-4-(2,3-dimethylphenyl)-3-hydroxypiperidine, 17 minutes. The identification o...
10.6084/m9.figshare.5104873.v1
null
Secondary alcohol.Secondary alcohol.Secondary amine
Ether.Secondary alcohol
c1ccccc1.C1CCNCC1.c1ccccc1.C1CCNCC1
c1ccccc1.C1CCNCC1
c1ccccc1.C1CCNCC1
Other
null
null
null
Cc1cccc([C@@H]2CCNC[C@@H]2O)c1C.Cc1cccc([C@H]2CCNC[C@H]2O)c1C>>Cc1cccc(OC2CCNCC2O)c1C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f9ddc22aff564f9bb539977507e82d66
Nc1c(Br)cc([N+](=O)[O-])cc1Br>>O=[N+]([O-])c1cc(Br)cc(Br)c1
BrC1=C(N)C(=CC(=C1)[N+](=O)[O-])Br.OS(=O)(=O)O.N(=O)[O-].[Na+]>>BrC1=CC(=CC(=C1)[N+](=O)[O-])Br
N[c:8]1[c:6]([Br:7])[cH:5][c:4]([N+:2](=[O:1])[O-:3])[cH:11][c:9]1[Br:10]>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][c:6]([Br:7])[cH:8][c:9]([Br:10])[cH:11]1
Nc1c(Br)cc([N+](=O)[O-])cc1Br
O=[N+]([O-])c1cc(Br)cc(Br)c1
null
null
C(C)O
Reduction
OtherReaction
a069304de6b46c6d557b2e80c544464adc3bb98001f26c098e87c25f29d552f9
a4f16f822d2806606c05d0c4baa1761ad37a11006840dde863a01a253bdff5dd
c1ccccc1
N-[c;H0;D3;+0:1](:[c:2](-[Br;D1;H0:3]):[c:4]):[c:5](-[Br;D1;H0:6]):[c:7]>>[Br;D1;H0:6]-[c:5](:[c:7]):[cH;D2;+0:1]:[c:2](-[Br;D1;H0:3]):[c:4]
93
[{"value": 93.0, "product": "BrC1=CC(=CC(=C1)[N+](=O)[O-])Br", "details": "PERCENTYIELD", "is_desired": false}, {"value": 92.8, "product": "BrC1=CC(=CC(=C1)[N+](=O)[O-])Br", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
(The named compound was synthesized according to Dumont, Bull. Soc. Chim. Bel., 505 (1995). This compound is also commercially available from Karl Industries, Aurora, Ohio.) To a suspension of 2,6-dibromo-4-nitroaniline (75.0 g, 254 mmol) in ethanol (1 L) was added H2SO4 (100 mL). The mixture was heated to reflux and s...
10.6084/m9.figshare.5104873.v1
null
Primary amine
null
c1ccccc1
c1ccccc1
c1ccccc1
Other
C(C)O
null
null
Nc1c(Br)cc([N+](=O)[O-])cc1Br>C(C)O>O=[N+]([O-])c1cc(Br)cc(Br)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e140c413254442d4bbef054ff1860151
CN(C)C(=O)N(C)C.O=[N+]([O-])c1cc(Br)cc(Br)c1.[OH-]>>Brc1cc(Br)cc(OCc2ccccc2)c1
BrC1=CC(=CC(=C1)[N+](=O)[O-])Br.[OH-].[K+].CN(C(N(C)C)=O)C>>BrC=1C=C(C=C(C1)Br)OCC1=CC=CC=C1
O=[C:2](N([CH3:7])[CH3:12])N([CH3:3])[CH3:14].O=[N+]([O-])[c:9]1[cH:6][c:4]([Br:5])[cH:15][c:10]([Br:1])[cH:11]1.[OH-:8]>>[Br:1][c:2]1[cH:3][c:4]([Br:5])[cH:6][c:7]([O:8][CH2:9][c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[cH:16]1
CN(C)C(=O)N(C)C.O=[N+]([O-])c1cc(Br)cc(Br)c1.[OH-]
Brc1cc(Br)cc(OCc2ccccc2)c1
null
[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC
null
Aromatic Heterocycle Formation
OtherReaction
39730c04ca2b5a982ac6a3a3e29fa56cee513216d32a08dffb9e06195509a888
7682ae28b24d6a4254d9e6cdb97956c47d58fd8b43dbcd58057fb712f57afb50
c1ccc(COc2ccccc2)cc1
O=[C;H0;D3;+0:1](-N(-[CH3;D1;+0:2])-[CH3;D1;+0:3])-N(-[CH3;D1;+0:4])-[CH3;D1;+0:5].O=[N+](-[O-])-[c;H0;D3;+0:6]1:[cH;D2;+0:7]:[c;H0;D3;+0:8](-[Br;H0;D1;+0:9]):[cH;D2;+0:10]:[c;H0;D3;+0:11](-[Br;D1;H0:12]):[cH;D2;+0:13]:1.[OH-;D0:14]>>[Br;D1;H0:12]-[c;H0;D3;+0:11]1:[cH;D2;+0:3]:[c;H0;D3;+0:1](-[Br;H0;D1;+0:9]):[c:15]:[c...
92
[{"value": 92.0, "product": "BrC=1C=C(C=C(C1)Br)OCC1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
6
HOUR
(According to Effenberger, Chem. Ber. 163 (1991).) 1,3-dibromo-5-nitrobenzene (2.81 g, 10.0 mmol), freshly powdered potassium hydroxide (1.00 g, 17.8 mmol) and tetrabutylammonium bromide (0.32 g, 1.00 mmol) were dissolved in tetramethyl urea (TMU, 8 mL). Oxygen was bubbled through the reaction mixture for 5 min and a s...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide.Urea.Nitro group
Aromatic halide.Aromatic halide.Ether
c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
HO-
[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC
null
6
CN(C)C(=O)N(C)C.O=[N+]([O-])c1cc(Br)cc(Br)c1.[OH-]>[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC>Brc1cc(Br)cc(OCc2ccccc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3d3acff8689841b194edf640c7e83d10
COc1ccc(CO)cc1.O=[N+]([O-])c1cc(Br)cc(Br)c1>>COc1ccc(COc2cc(Br)cc(Br)c2)cc1
COC=1C=CC(=CC1)CO.BrC1=CC(=CC(=C1)[N+](=O)[O-])Br.[OH-].[K+]>>BrC=1C=C(C=C(C1)Br)OCC1=CC=C(C=C1)OC
[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][OH:8])[cH:17][cH:18]1.O=[N+]([O-])[c:9]1[cH:10][c:11]([Br:12])[cH:13][c:14]([Br:15])[cH:16]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][O:8][c:9]2[cH:10][c:11]([Br:12])[cH:13][c:14]([Br:15])[cH:16]2)[cH:17][cH:18]1
COc1ccc(CO)cc1.O=[N+]([O-])c1cc(Br)cc(Br)c1
COc1ccc(COc2cc(Br)cc(Br)c2)cc1
null
[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC
CN(C(N(C)C)=O)C
Functional Group Interconversion
OtherReaction
585e0ff0de8fd5f82bfaab47faba0014fb24285662aa50a5e33791db94cefd4b
3990f9215b5a078e088ba5bbd0b8243e92e0f699f4ee1f20fbddffff29ec99ce
c1ccc(COc2ccccc2)cc1
O=[N+](-[O-])-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[OH;D1;+0:6]-[C:7]-[c:8]>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[O;H0;D2;+0:6]-[C:7]-[c:8]):[c:4]:[c:5]
74.4
[{"value": 74.4, "product": "BrC=1C=C(C=C(C1)Br)OCC1=CC=C(C=C1)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
48
HOUR
1,3-dibromo-5-nitrobenzene (30.0 g, 107 mmol), freshly powdered potassium hydroxide (10.8 g, 192 mmol) and tetrabutylammonium bromide (3.42 g, 10.7 mmol) were dissolved in tetramethyl urea (TMU, 90 mL). A solution of p-methoxybenzyl alcohol (17.8 g, 128 mmol) in TMU (30 mL) was added drop-wise at room temperature over ...
10.6084/m9.figshare.5104873.v1
null
Nitro group.Primary alcohol
Ether
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1
HO-
[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC.CN(C(N(C)C)=O)C
null
48
COc1ccc(CO)cc1.O=[N+]([O-])c1cc(Br)cc(Br)c1>[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC.CN(C(N(C)C)=O)C>COc1ccc(COc2cc(Br)cc(Br)c2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-eb7f12fb6a90449b92cf25742e870b2d
Brc1cc(Br)cc(OCc2ccccc2)c1.Nc1cccnc1>>Brc1cc(Nc2cccnc2)cc(OCc2ccccc2)c1
CCOC(=O)C.CCCCCCC.BrC=1C=C(C=C(C1)Br)OCC1=CC=CC=C1.NC=1C=NC=CC1.CC(C)([O-])C.[Na+]>>C(C1=CC=CC=C1)OC=1C=C(C=C(C1)Br)NC=1C=NC=CC1
Br[c:4]1[cH:3][c:2]([Br:1])[cH:22][c:13]([O:14][CH2:15][c:16]2[cH:17][cH:18][cH:19][cH:20][cH:21]2)[cH:12]1.[NH2:5][c:6]1[cH:7][cH:8][cH:9][n:10][cH:11]1>>[Br:1][c:2]1[cH:3][c:4]([NH:5][c:6]2[cH:7][cH:8][cH:9][n:10][cH:11]2)[cH:12][c:13]([O:14][CH2:15][c:16]2[cH:17][cH:18][cH:19][cH:20][cH:21]2)[cH:22]1
Brc1cc(Br)cc(OCc2ccccc2)c1.Nc1cccnc1
Brc1cc(Nc2cccnc2)cc(OCc2ccccc2)c1
null
C1=CC=C(C=C1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C1=CC=C(C=C1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C1=CC=C(C=C1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C(Cl)(Cl)Cl.[Pd].[Pd]
C1(=CC=CC=C1)C.[Cl-].[Na+].O
Heteroatom Alkylation and Arylation
N-arylation (Buchwald-Hartwig/Ullmann-Goldberg)
da9dae6a655c4bd18887b692f91621e77027436294d6e1fc7be7295afb364796
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(COc2cccc(Nc3cccnc3)c2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]:[c:11]>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]:[c:11]):[c:4]:[c:5]
41
[{"value": 41.0, "product": "C(C1=CC=CC=C1)OC=1C=C(C=C(C1)Br)NC=1C=NC=CC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 40.5, "product": "C(C1=CC=CC=C1)OC=1C=C(C=C(C1)Br)NC=1C=NC=CC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
85
CELSIUS
10
MINUTE
An oven-dried flask was charged with (±)-BINAP (1.05 g, 1.68 mmol), Pd2(dba)3 CHCl3-complex (580 mg, 0.56 mmol) and then flushed with argon. Degassed toluene (28 mL) was added and the solution was stirred for 10 min. The catalyst solution was added to a mixture of 3,5-dibromo-1-benzyloxybenzene (38.3 g, 112 mmol), 3-am...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ccccc1
c1ccccc1
c1ccccc1.c1ccncc1.c1ccccc1
HBr
C1=CC=C(C=C1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C1=CC=C(C=C1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C1=CC=C(C=C1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C(Cl)(Cl)Cl.[Pd].[Pd].C1(=CC=CC=C1)C.[Cl-].[Na+].O
85
0.166667
Brc1cc(Br)cc(OCc2ccccc2)c1.Nc1cccnc1>C1=CC=C(C=C1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C1=CC=C(C=C1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C1=CC=C(C=C1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C(Cl)(Cl)Cl.[Pd].[Pd].C1(=CC=CC=C1)C.[Cl-].[Na+].O>Brc1cc(Nc2cccnc2)cc(OCc2ccccc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9655981e253346789505a2b9054eb072
COc1ccc(COc2cc(Br)cc(Br)c2)cc1.Nc1cccnc1>>COc1ccc(COc2cc(Br)cc(Nc3cccnc3)c2)cc1
CCOC(=O)C.BrC=1C=C(C=C(C1)Br)OCC1=CC=C(C=C1)OC.NC=1C=NC=CC1.C(C)(C)(C)[O-].[Na+]>>COC1=CC=C(COC=2C=C(C=C(C2)Br)NC=2C=NC=CC2)C=C1
Br[c:14]1[cH:13][c:11]([Br:12])[cH:10][c:9]([O:8][CH2:7][c:6]2[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:24][cH:23]2)[cH:22]1.[NH2:15][c:16]1[cH:17][cH:18][cH:19][n:20][cH:21]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][O:8][c:9]2[cH:10][c:11]([Br:12])[cH:13][c:14]([NH:15][c:16]3[cH:17][cH:18][cH:19][n:20][cH:21]3)[cH:22]2)[...
COc1ccc(COc2cc(Br)cc(Br)c2)cc1.Nc1cccnc1
COc1ccc(COc2cc(Br)cc(Nc3cccnc3)c2)cc1
null
C1=CC=C(C=C1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C1=CC=C(C=C1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C1=CC=C(C=C1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C(Cl)(Cl)Cl.[Pd].[Pd]
CCOC(=O)C.CCCCCCC.C1(=CC=CC=C1)C.[Cl-].[Na+].O
Heteroatom Alkylation and Arylation
N-arylation (Buchwald-Hartwig/Ullmann-Goldberg)
da9dae6a655c4bd18887b692f91621e77027436294d6e1fc7be7295afb364796
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(COc2cccc(Nc3cccnc3)c2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]:[c:11]>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]:[c:11]):[c:4]:[c:5]
75
[{"value": 75.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
90
CELSIUS
10
MINUTE
An oven-dried flask was charged with (±)-BINAP (504 mg, 0.81 mmol), Pd2(dba)3 CHCl3-complex (278 mg, 0.27 mmol) and then flushed with argon. Degassed toluene (50 mL) was added and the solution was stirred for 10 min. A second oven-dried flask was charged with 3,5-dibromo-1-p-methoxy-benzyloxybenzene (20.0 g, 53.8 mmol)...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1.c1ccncc1
HBr
C1=CC=C(C=C1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C1=CC=C(C=C1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C1=CC=C(C=C1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C(Cl)(Cl)Cl.[Pd].[Pd].CCOC(=O)C.CCCCCCC.C1(=CC=CC=C1)C.[Cl-].[Na+].O
90
0.166667
COc1ccc(COc2cc(Br)cc(Br)c2)cc1.Nc1cccnc1>C1=CC=C(C=C1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C1=CC=C(C=C1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C1=CC=C(C=C1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C(Cl)(Cl)Cl.[Pd].[Pd].CCOC(=O)C.CCCCCCC.C1(=CC=CC=C1)C.[Cl-].[Na+].O>COc1ccc(COc2cc(Br)cc(Nc3cccnc3)c2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-582ddb996ddd4c0bb4300f2ed1efe680
COc1ccc(COc2cc(Nc3cccnc3)cc(-c3cccc4sccc34)c2)cc1>>Oc1cc(Nc2cccnc2)cc(-c2cccc3sccc23)c1
S1C2=C(C=C1)C(=CC=C2)C=2C=C(C=C(C2)OCC2=CC=C(C=C2)OC)NC=2C=NC=CC2.C1(=CC=CC=C1)SC.FC(C(=O)O)(F)F>>S1C2=C(C=C1)C(=CC=C2)C=2C=C(C=C(C2)NC=2C=NC=CC2)O
COc1ccc(C[O:1][c:2]2[cH:3][c:4]([NH:5][c:6]3[cH:7][cH:8][cH:9][n:10][cH:11]3)[cH:12][c:13](-[c:14]3[cH:15][cH:16][cH:17][c:18]4[s:19][cH:20][cH:21][c:22]34)[cH:23]2)cc1>>[OH:1][c:2]1[cH:3][c:4]([NH:5][c:6]2[cH:7][cH:8][cH:9][n:10][cH:11]2)[cH:12][c:13](-[c:14]2[cH:15][cH:16][cH:17][c:18]3[s:19][cH:20][cH:21][c:22]23)[c...
COc1ccc(COc2cc(Nc3cccnc3)cc(-c3cccc4sccc34)c2)cc1
Oc1cc(Nc2cccnc2)cc(-c2cccc3sccc23)c1
null
null
C(Cl)Cl
Reduction
OtherReaction
8a4606e79840bb3d9b3a2e0b7d9ed5648d76ae6cbcc894506db9722ac2624f9a
3165f563067f8d27bb50b0da034e3e854d1ead7f745de7cf575f7ca4cf677789
c1cncc(Nc2cccc(-c3cccc4sccc34)c2)c1
C-O-c1:c:c:c(-C-[O;H0;D2;+0:1]-[c:2](:[c:3]):[c:4]):c:c:1>>[OH;D1;+0:1]-[c:2](:[c:3]):[c:4]
66.7
[{"value": 58.0, "product": "S1C2=C(C=C1)C(=CC=C2)C=2C=C(C=C(C2)NC=2C=NC=CC2)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 66.7, "product": "S1C2=C(C=C1)C(=CC=C2)C=2C=C(C=C(C2)NC=2C=NC=CC2)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
5
HOUR
[3-benzo[b]thiophen-4-yl-5-(4-methoxy-benzyloxy)-phenyl]-pyridin-3-yl-amine (35 mg, 0.08 mmol) was dissolved in CH2Cl2 (1 mL) and thioanisole (188 μL, 1.60 mmol) was added. The solution was cooled to 0° C. and trifluoroacetic acid (0.1 mL) was added. The reaction mixture was stirred at room temperature for 5 h and was ...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether
Aromatic alcohol
c1ccccc1
null
c1ccccc1.c1ccncc1.c1ccc2sccc2c1
HO-
C(Cl)Cl
0
5
COc1ccc(COc2cc(Nc3cccnc3)cc(-c3cccc4sccc34)c2)cc1>C(Cl)Cl>Oc1cc(Nc2cccnc2)cc(-c2cccc3sccc23)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ded46bef1bef45f9a82d0d90149d9313
COc1ccc(Cc2cc(Br)cc(Nc3cccnc3)c2)cc1.O=[N+]([O-])c1ccc2cc[nH]c2c1>>O=[N+]([O-])c1ccc2ccn(-c3cc(O)cc(Nc4cccnc4)c3)c2c1
P(=O)([O-])([O-])[O-].[K+].[K+].[K+].[N+](=O)([O-])C1=CC=C2C=CNC2=C1.CNCCNC.BrC=1C=C(C=C(C1)CC1=CC=C(C=C1)OC)NC=1C=NC=CC1>>[N+](=O)([O-])C1=CC=C2C=CN(C2=C1)C=1C=C(C=C(C1)NC=1C=NC=CC1)O
C[O:14]c1ccc(C[c:11]2[cH:12][c:13](Br)[cH:15][c:16]([NH:17][c:18]3[cH:19][cH:20][cH:21][n:22][cH:23]3)[cH:24]2)cc1.[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]2[cH:8][cH:9][nH:10][c:25]2[cH:26]1>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]2[cH:8][cH:9][n:10](-[c:11]3[cH:12][c:13]([OH:14])[cH:15][c:16]([NH:17][c:18]4[cH:...
COc1ccc(Cc2cc(Br)cc(Nc3cccnc3)c2)cc1.O=[N+]([O-])c1ccc2cc[nH]c2c1
O=[N+]([O-])c1ccc2ccn(-c3cc(O)cc(Nc4cccnc4)c3)c2c1
null
[Cu]I
C1(=CC=CC=C1)C.C(Cl)Cl
Functional Group Addition
OtherReaction
a32afc24d96451c382dc4201082b19044aee20ea0e571d31f34af06c379170ae
8a5089a4a46e8f89fdbb977c3fed3a2378e3bcd5a197b8cfa9ddc8a8a34b2a51
c1cncc(Nc2cccc(-n3ccc4ccccc43)c2)c1
Br-[c;H0;D3;+0:1]1:[c:2]:[c;H0;D3;+0:3](-C-c2:c:c:c(-[O;H0;D2;+0:4]-C):c:c:2):[c:5]:[c:6]:[c:7]:1.[c:8]:[c:9]1:[c:10]:[c:11]:[c:12]:[nH;D2;+0:13]:1>>[OH;D1;+0:4]-[c;H0;D3;+0:1]1:[c:2]:[c;H0;D3;+0:3](-[n;H0;D3;+0:13]2:[c:12]:[c:11]:[c:10]:[c:9]:2:[c:8]):[c:5]:[c:6]:[c:7]:1
null
[]
110
CELSIUS
null
null
The resin-bound (3-bromo-5-p-methoxybenzylphenyl)-3-pyridylamine described in Example 22 (200 mg, ca 0.12 mmol) was placed in a 50 mL glass reactor. Copper (I) iodide (0.6 mmol, 114 mg), potassium phosphate (127 mg, 0.6 mmol), toluene (5 mL), 6-nitroindole (0.6 mmol, 98 mg) and N,N′-dimethylethylenediamine (53 mg, 0.6 ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ether
Aromatic alcohol
c1ccccc1.c1ccccc1.c1ccc2[nH]ccc2c1
c1ccc2cc[nH]c2c1.c1ccccc1
c1ccc2cc[nH]c2c1.c1ccccc1.c1ccncc1
HBr
[Cu]I.C1(=CC=CC=C1)C.C(Cl)Cl
110
null
COc1ccc(Cc2cc(Br)cc(Nc3cccnc3)c2)cc1.O=[N+]([O-])c1ccc2cc[nH]c2c1>[Cu]I.C1(=CC=CC=C1)C.C(Cl)Cl>O=[N+]([O-])c1ccc2ccn(-c3cc(O)cc(Nc4cccnc4)c3)c2c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f204a4fc1199400a9a77315d8cc9ea00
COc1ccc(COc2cc(C(=O)c3cccnc3)cc(-c3cccc4c3ccn4[Si](C(C)C)(C(C)C)C(C)C)c2)cc1.NO>>COc1ccc(COc2cc(C(=NO)c3cccnc3)cc(-c3cccc4c3ccn4[Si](C(C)C)(C(C)C)C(C)C)c2)cc1
COC1=CC=C(COC=2C=C(C=C(C2)C2=C3C=CN(C3=CC=C2)[Si](C(C)C)(C(C)C)C(C)C)C(=O)C=2C=NC=CC2)C=C1.Cl.ON>>COC1=CC=C(COC=2C=C(C=C(C2)C2=C3C=CN(C3=CC=C2)[Si](C(C)C)(C(C)C)C(C)C)C(=NO)C=2C=NC=CC2)C=C1
O=[C:12]([c:11]1[cH:10][c:9]([O:8][CH2:7][c:6]2[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:44][cH:43]2)[cH:42][c:22](-[c:23]2[cH:24][cH:25][cH:26][c:27]3[c:28]2[cH:29][cH:30][n:31]3[Si:32]([CH:33]([CH3:34])[CH3:35])([CH:36]([CH3:37])[CH3:38])[CH:39]([CH3:40])[CH3:41])[cH:21]1)[c:15]1[cH:16][cH:17][cH:18][n:19][cH:20]1.[NH2:13][...
COc1ccc(COc2cc(C(=O)c3cccnc3)cc(-c3cccc4c3ccn4[Si](C(C)C)(C(C)C)C(C)C)c2)cc1.NO
COc1ccc(COc2cc(C(=NO)c3cccnc3)cc(-c3cccc4c3ccn4[Si](C(C)C)(C(C)C)C(C)C)c2)cc1
null
null
C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
b5fd91d879f097d0ef2e8e2d3ef7d2ef0195968870a9602a47b8324c601790b9
1a0ef15294bdb221fb8888b5d4c7fcf00473b11e53da288791d32747daa48d23
N=C(c1cccnc1)c1cc(OCc2ccccc2)cc(-c2cccc3[nH]ccc23)c1
O=[C;H0;D3;+0:1](-[c:2](:[c:3]):[c:4])-[c:5](:[c:6]):[c:7]:[#7;a:8]:[c:9].[NH2;D1;+0:10]-[O;D1;H1:11]>>[O;D1;H1:11]-[N;H0;D2;+0:10]=[C;H0;D3;+0:1](-[c:2](:[c:3]):[c:4])-[c:5](:[c:6]):[c:7]:[#7;a:8]:[c:9]
null
[]
null
null
2
HOUR
[3-(4-methoxy-benzyloxy)-5-(1-triisopropylsilanyl-1H-indol-4-yl)-phenyl]-pyridin-3-yl-methanone (50 mg, 0.085 mmol) and hydroxyamine hydrochloride (29 mg, 0.42 mmol) in 2 mL of ethanol was heated to reflux. After 2 hrs, the reaction was completed. The solvent was removed under reduced pressure. The crude product was re...
10.6084/m9.figshare.5104873.v1
null
Ketone.Primary amine
Oxime
null
null
c1ccccc1.c1ccccc1.c1ccncc1.c1cccc2[nH]ccc12
HO-
C(C)O
null
2
COc1ccc(COc2cc(C(=O)c3cccnc3)cc(-c3cccc4c3ccn4[Si](C(C)C)(C(C)C)C(C)C)c2)cc1.NO>C(C)O>COc1ccc(COc2cc(C(=NO)c3cccnc3)cc(-c3cccc4c3ccn4[Si](C(C)C)(C(C)C)C(C)C)c2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8c2653f0cac1492cbf088944d2dd581a
CC(C)[Si](C(C)C)(C(C)C)n1ccc2c(-c3cc(OCc4ccccc4)nc(Nc4cccnc4)n3)cccc21>>Oc1cc(-c2cccc3[nH]ccc23)nc(Nc2cccnc2)n1
C(C1=CC=CC=C1)OC1=NC(=NC(=C1)C1=C2C=CN(C2=CC=C1)[Si](C(C)C)(C(C)C)C(C)C)NC=1C=NC=CC1.C(C1=CC=CC=C1)OC1=NC(=NC(=C1)Cl)NC=1C=NC=CC1.C([O-])([O-])=O.[K+].[K+].CC1(OB(OC1(C)C)C1=C2C=CN(C2=CC=C1)[Si](C(C)C)(C(C)C)C(C)C)C>>N1C=CC2=C(C=CC=C12)C1=CC(=NC(=N1)NC=1C=NC=CC1)O
CC(C)[Si](C(C)C)(C(C)C)[n:10]1[c:9]2[cH:8][cH:7][cH:6][c:5](-[c:4]3[cH:3][c:2]([O:1]Cc4ccccc4)[n:23][c:15]([NH:16][c:17]4[cH:18][cH:19][cH:20][n:21][cH:22]4)[n:14]3)[c:13]2[cH:12][cH:11]1>>[OH:1][c:2]1[cH:3][c:4](-[c:5]2[cH:6][cH:7][cH:8][c:9]3[nH:10][cH:11][cH:12][c:13]23)[n:14][c:15]([NH:16][c:17]2[cH:18][cH:19][cH:2...
CC(C)[Si](C(C)C)(C(C)C)n1ccc2c(-c3cc(OCc4ccccc4)nc(Nc4cccnc4)n3)cccc21
Oc1cc(-c2cccc3[nH]ccc23)nc(Nc2cccnc2)n1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O1CCOCC1.CN(C)C=O
Deprotection
OtherReaction
495cb76f602ebd19a8a5962d26b650b172d6ae8b0c11815bbf9f60e06b9b1e13
5e40339a4a04757b519e3c89ecb7b8ce3defd2e5e05bc91c5ac27f57100aee42
c1cncc(Nc2nccc(-c3cccc4[nH]ccc34)n2)c1
C(-[O;H0;D2;+0:1]-[c:2]1:[#7;a:3]:[c:4]:[#7;a:5]:[c:6]:[c:7]:1)-c1:c:c:c:c:c:1.C-C(-C)-[Si](-C(-C)-C)(-C(-C)-C)-[n;H0;D3;+0:8]1:[c:9]:[c:10]:[c:11]:[c:12]:1:[c:13]>>[OH;D1;+0:1]-[c:2]1:[#7;a:3]:[c:4]:[#7;a:5]:[c:6]:[c:7]:1.[c:13]:[c:12]1:[c:11]:[c:10]:[c:9]:[nH;D2;+0:8]:1
null
[]
null
null
null
null
[4-Benzyloxy-6-(1-triisopropylsilanyl-1H-indol-4-yl)-pyrimidin-2-yl]-pyridin-3-yl-amine. DMF (1 mL) and dioxane (2 mL) were added through a septum to a nitrogen-purged microwave tube containing (4-benzyloxy-6-chloro-pyrimidin-2-yl)-pyridin-3-yl-amine (80 mg, 0.256 mmol), potassium carbonate (71 mg, 0.50 mmol), Pd(PPh3)...
10.6084/m9.figshare.5104873.v1
null
Ether.Silyl protective group
Aromatic alcohol
c1cccc2[nH]ccc12.c1ccccc1
c1ccc2[nH]ccc2c1
c1cncnc1.c1ccc2[nH]ccc2c1.c1ccncc1
Other
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1.CN(C)C=O
null
null
CC(C)[Si](C(C)C)(C(C)C)n1ccc2c(-c3cc(OCc4ccccc4)nc(Nc4cccnc4)n3)cccc21>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O1CCOCC1.CN(C)C=O>Oc1cc(-c2cccc3[nH]ccc23)nc(Nc2cccnc2)n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4d26c78cbdef44779b108ae6e7f26c9c
COc1ccc(COc2cc(Br)cc(Nc3cccnc3)c2)cc1.N#Cc1ccc2[nH]ccc2c1>>N#Cc1ccc2c(ccn2-c2cc(O)cc(Nc3cccnc3)c2)c1
BrC=1C=C(C=C(C1)OCC1=CC=C(C=C1)OC)NC=1C=NC=CC1.P(=O)([O-])([O-])[O-].[K+].[K+].[K+].C(#N)C=1C=C2C=CNC2=CC1.CNCCNC>>OC=1C=C(C=C(C1)NC=1C=NC=CC1)N1C=CC2=CC(=CC=C12)C#N
COc1ccc(C[O:14][c:13]2[cH:12][c:11](Br)[cH:24][c:16]([NH:17][c:18]3[cH:19][cH:20][cH:21][n:22][cH:23]3)[cH:15]2)cc1.[N:1]#[C:2][c:3]1[cH:4][cH:5][c:6]2[c:7]([cH:8][cH:9][nH:10]2)[cH:25]1>>[N:1]#[C:2][c:3]1[cH:4][cH:5][c:6]2[c:7]([cH:8][cH:9][n:10]2-[c:11]2[cH:12][c:13]([OH:14])[cH:15][c:16]([NH:17][c:18]3[cH:19][cH:20]...
COc1ccc(COc2cc(Br)cc(Nc3cccnc3)c2)cc1.N#Cc1ccc2[nH]ccc2c1
N#Cc1ccc2c(ccn2-c2cc(O)cc(Nc3cccnc3)c2)c1
null
[Cu]I
C1(=CC=CC=C1)C
Heteroatom Alkylation and Arylation
OtherReaction
8246b8e0885ddf770fb4c8d79c1e3f38929caaa2e872d869c6b0b455195b8f06
c3e82c812dc6c78070ba1f75e08effdbeaff4cd50c4337e2c1365f20b4956654
c1cncc(Nc2cccc(-n3ccc4ccccc43)c2)c1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[O;H0;D2;+0:4]-C-c2:c:c:c(-O-C):c:c:2):[c:5]:[c:6]:[c:7]:1.[c:8]:[c:9]1:[c:10]:[c:11]:[c:12]:[nH;D2;+0:13]:1>>[OH;D1;+0:4]-[c:3]1:[c:2]:[c;H0;D3;+0:1](-[n;H0;D3;+0:13]2:[c:12]:[c:11]:[c:10]:[c:9]:2:[c:8]):[c:7]:[c:6]:[c:5]:1
10.8
[{"value": 10.8, "product": "OC=1C=C(C=C(C1)NC=1C=NC=CC1)N1C=CC2=CC(=CC=C12)C#N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
110
CELSIUS
null
null
[3-Bromo-5-(4-methoxy-benzyloxy)-phenyl]-pyridin-3-yl-amine (193 mg, ca 0.5 mmol) was placed in a 5 mL glass reactor. Copper (I) iodide (0.5 mmol, 96 mg), potassium phosphate (213 mg, 1 mmol), toluene (3 mL), 5-cyanoindole (1.0 mmol, 142 mg) and N,N′-dimethylethylenediamine (53 mg, 0.6 mmol) were added to the reactor, ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ether.Ether
Aromatic alcohol
c1ccccc1.c1ccccc1.c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1.c1ccncc1
HBr
[Cu]I.C1(=CC=CC=C1)C
110
null
COc1ccc(COc2cc(Br)cc(Nc3cccnc3)c2)cc1.N#Cc1ccc2[nH]ccc2c1>[Cu]I.C1(=CC=CC=C1)C>N#Cc1ccc2c(ccn2-c2cc(O)cc(Nc3cccnc3)c2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-931461be7229496e836defd5785e4db4
COc1ccc(COc2cc(Br)cc(Br)c2)cc1.COc1ccc(COc2cc(Br)cc(Nc3ccc(OCc4ccccc4)nc3)c2)cc1>>COc1ccc(COc2cc(N)cc(Br)c2)cc1
C(C1=CC=CC=C1)OC1=CC=C(C=N1)N.BrC1=CC(=CC(=C1)OCC1=CC=C(C=C1)OC)Br.CC(C)(C)[O-].[Na+].C(C1=CC=CC=C1)OC1=CC=C(C=N1)NC1=CC(=CC(=C1)OCC1=CC=C(C=C1)OC)Br>>BrC=1C=C(C=C(C1)OCC1=CC=C(C=C1)OC)N
Br[c:11]1[cH:10][c:9]([O:8][CH2:7][c:6]2[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:18][cH:17]2)[cH:16][c:14]([Br:15])[cH:13]1.COc1ccc(COc2cc(Br)cc([NH:12]c3ccc(OCc4ccccc4)nc3)c2)cc1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][O:8][c:9]2[cH:10][c:11]([NH2:12])[cH:13][c:14]([Br:15])[cH:16]2)[cH:17][cH:18]1
COc1ccc(COc2cc(Br)cc(Br)c2)cc1.COc1ccc(COc2cc(Br)cc(Nc3ccc(OCc4ccccc4)nc3)c2)cc1
COc1ccc(COc2cc(N)cc(Br)c2)cc1
null
C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd].C=1C=CC(=CC1)P(C=2C=CC=CC2)C3=CC=C4C=CC=CC4=C3C5=C6C=CC=CC6=CC=C5P(C=7C=CC=CC7)C=8C=CC=CC8
null
Heteroatom Alkylation and Arylation
OtherReaction
285d763a51f37794cdad66c72d48d0d44a3fcbc0fdf73d0fca473c1c998f6180
f9b3fc120e1f63fc61f4091f79b5f0d58358f7d72db88a5e5844c6ed41e6a76b
c1ccc(COc2ccccc2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].Br-c1:c:c(-O-C-c2:c:c:c(-O-C):c:c:2):c:c(-[NH;D2;+0:6]-c2:c:c:c(-O-C-c3:c:c:c:c:c:3):n:c:2):c:1>>[NH2;D1;+0:6]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
47
[{"value": 47.0, "product": "BrC=1C=C(C=C(C1)OCC1=CC=C(C=C1)OC)N", "details": "PERCENTYIELD", "is_desired": false}]
120
CELSIUS
null
null
(6-benzyloxy-pyridin-3-yl)-[3-bromo-5-(4-methoxy-benzyloxy)-phenyl]-amine. A dry tube was charged with 6-benzyloxy-pyridin-3-ylamine (68 mg, 0.34 mmol), 1,3-dibromo-5-(4-methoxy-benzyloxy)-benzene (126 mg, 0.34 mmol), NaOtBu (46 mg, 0.48 mmol), Pd2(dba)3 (3.1 mg, 0.0034 mmol), BINAP (6.3 mg, 0.01 mmol) and degassed tol...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide.Ether.Ether.Ether.Secondary amine
Primary amine
c1ccccc1.c1ccccc1.c1ccccc1.c1ccncc1.c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1
HBr
C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd].C=1C=CC(=CC1)P(C=2C=CC=CC2)C3=CC=C4C=CC=CC4=C3C5=C6C=CC=CC6=CC=C5P(C=7C=CC=CC7)C=8C=CC=CC8
120
null
COc1ccc(COc2cc(Br)cc(Br)c2)cc1.COc1ccc(COc2cc(Br)cc(Nc3ccc(OCc4ccccc4)nc3)c2)cc1>C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd].C=1C=CC(=CC1)P(C=2C=CC=CC2)C3=CC=C4C=CC=CC4=C3C5=C6C=CC=CC6=CC=C5P(C=7C=CC=CC7)C=8C=CC=CC8>COc1ccc(COc2cc(N)c...
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0d8a05038e0b418682bb41b4051f3946
CC(C)[Si](C(C)C)(C(C)C)n1ccc2c(B3OC(C)(C)C(C)(C)O3)cccc21.COc1ccc(COc2cc(Br)cc(Nc3ccc(OCc4ccccc4)nc3)c2)cc1>>Oc1cc(Nc2cccnc2O)cc(-c2cccc3[nH]ccc23)c1
C(C1=CC=CC=C1)OC1=CC=C(C=N1)NC1=CC(=CC(=C1)OCC1=CC=C(C=C1)OC)Br.CC1(OB(OC1(C)C)C1=C2C=CN(C2=CC=C1)[Si](C(C)C)(C(C)C)C(C)C)C.[O-]P(=O)([O-])[O-].[K+].[K+].[K+].C(C1=CC=CC=C1)OC1=CC=C(C=N1)NC1=CC(=CC(=C1)C1=C2C=CN(C2=CC=C1)[Si](C(C)C)(C(C)C)C(C)C)OCC1=CC=C(C=C1)OC>>OC=1C=C(C=C(C1)C1=C2C=CNC2=CC=C1)NC=1C(=NC=CC1)O
CC(C)[Si](C(C)C)(C(C)C)[n:20]1[c:19]2[cH:18][cH:17][cH:16][c:15](B3OC(C)(C)C(C)(C)O3)[c:23]2[cH:22][cH:21]1.COc1ccc(C[O:1][c:2]2[cH:3][c:4]([NH:5][c:6]3[cH:7][cH:8][c:9]([O:12]Cc4ccccc4)[n:10][cH:11]3)[cH:13][c:14](Br)[cH:24]2)cc1>>[OH:1][c:2]1[cH:3][c:4]([NH:5][c:6]2[cH:7][cH:8][cH:9][n:10][c:11]2[OH:12])[cH:13][c:14]...
CC(C)[Si](C(C)C)(C(C)C)n1ccc2c(B3OC(C)(C)C(C)(C)O3)cccc21.COc1ccc(COc2cc(Br)cc(Nc3ccc(OCc4ccccc4)nc3)c2)cc1
Oc1cc(Nc2cccnc2O)cc(-c2cccc3[nH]ccc23)c1
null
Cl[Pd-](C1=C(C=CC=C1)C1=C(C=CC=C1)N(C)C)P(C1C2CCC(C1)C2)C2C1CCC(C2)C1
O1CCOCC1
Heteroatom Alkylation and Arylation
OtherReaction
db8d541dfd7dc38b3b8482e14552e3171bc48f887dfd400dc975b9e9e284c679
199f12599629136c735d0ade11f454f145e4cbfd03347490ea78984a0acd7720
c1cncc(Nc2cccc(-c3cccc4[nH]ccc34)c2)c1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[#7:4]-[c:5]2:[c:6]:[c:7]:[c;H0;D3;+0:8](-[O;H0;D2;+0:9]-C-c3:c:c:c:c:c:3):[#7;a:10]:[cH;D2;+0:11]:2):[c:12]:[c:13](-[O;H0;D2;+0:14]-C-c2:c:c:c(-O-C):c:c:2):[c:15]:1.C-C(-C)-[Si](-C(-C)-C)(-C(-C)-C)-[n;H0;D3;+0:16]1:[c:17]:[c:18]:[c:19]2:[c:20]:1:[c:21]:[c:22]:[c:23]:[c;H0;D3;+0:24]:2-B1...
57.1
[{"value": 57.1, "product": "OC=1C=C(C=C(C1)C1=C2C=CNC2=CC=C1)NC=1C(=NC=CC1)O", "details": "PERCENTYIELD", "is_desired": false}]
120
CELSIUS
null
null
(6-benzyloxy-pyridin-3-yl)-[3-(4-methoxy-benzyloxy)-5-(1-triisopropylsilanyl-1H-indol-4-yl)-phenyl]-amine. To a tube purged with nitrogen containing (6-benzyloxy-pyridin-3-yl)-[3-bromo-5-(4-methoxy-benzyloxy)-phenyl]-amine (78 mg, 0.158 mmol), 4-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-1-triisopropylsilanyl-1H-in...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ether.Ether.Ether.Boronic ester.Silyl protective group
Aromatic alcohol.Aromatic alcohol
c1cccc2[nH]ccc12.B1OCCO1.c1ccccc1.c1ccccc1.c1ccncc1.c1ccccc1
c1ccccc1.c1ccncc1.c1ccc2[nH]ccc2c1
c1ccccc1.c1ccncc1.c1ccc2[nH]ccc2c1
HBr.B
Cl[Pd-](C1=C(C=CC=C1)C1=C(C=CC=C1)N(C)C)P(C1C2CCC(C1)C2)C2C1CCC(C2)C1.O1CCOCC1
120
null
CC(C)[Si](C(C)C)(C(C)C)n1ccc2c(B3OC(C)(C)C(C)(C)O3)cccc21.COc1ccc(COc2cc(Br)cc(Nc3ccc(OCc4ccccc4)nc3)c2)cc1>Cl[Pd-](C1=C(C=CC=C1)C1=C(C=CC=C1)N(C)C)P(C1C2CCC(C1)C2)C2C1CCC(C2)C1.O1CCOCC1>Oc1cc(Nc2cccnc2O)cc(-c2cccc3[nH]ccc23)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f8d0d240a83c41eda633c9e7bf13f4cc
CC(C)[Si](C(C)C)(C(C)C)n1ccc2c(-c3cc(O)cc(Nc4ccc(O)nc4)c3)cccc21>>Oc1cc(Nc2ccc(O)nc2)cc(-c2cccc3[nH]ccc23)c1
OC=1C=C(C=C(C1)C1=C2C=CN(C2=CC=C1)[Si](C(C)C)(C(C)C)C(C)C)NC=1C=CC(=NC1)O>>OC=1C=C(C=C(C1)C1=C2C=CNC2=CC=C1)NC=1C=CC(=NC1)O
CC(C)[Si](C(C)C)(C(C)C)[n:20]1[c:19]2[cH:18][cH:17][cH:16][c:15](-[c:14]3[cH:13][c:4]([NH:5][c:6]4[cH:7][cH:8][c:9]([OH:10])[n:11][cH:12]4)[cH:3][c:2]([OH:1])[cH:24]3)[c:23]2[cH:22][cH:21]1>>[OH:1][c:2]1[cH:3][c:4]([NH:5][c:6]2[cH:7][cH:8][c:9]([OH:10])[n:11][cH:12]2)[cH:13][c:14](-[c:15]2[cH:16][cH:17][cH:18][c:19]3[n...
CC(C)[Si](C(C)C)(C(C)C)n1ccc2c(-c3cc(O)cc(Nc4ccc(O)nc4)c3)cccc21
Oc1cc(Nc2ccc(O)nc2)cc(-c2cccc3[nH]ccc23)c1
null
null
C(=O)(C(F)(F)F)O.C(Cl)Cl
Deprotection
OtherReaction
7c2e21594486284c07d91d3a35172f6f97c1f0e21d7ef6570d737987b23577df
97c217b2f55def3964724d0808498dda438b599ce2ff7b0e4e056e4419d08380
c1cncc(Nc2cccc(-c3cccc4[nH]ccc34)c2)c1
C-C(-C)-[Si](-C(-C)-C)(-C(-C)-C)-[n;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[c:5]:1:[c:6]>>[c:6]:[c:5]1:[c:4]:[c:3]:[c:2]:[nH;D2;+0:1]:1
1.5
[{"value": 1.5, "product": "OC=1C=C(C=C(C1)C1=C2C=CNC2=CC=C1)NC=1C=CC(=NC1)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 1.5, "product": "OC=1C=C(C=C(C1)C1=C2C=CNC2=CC=C1)NC=1C=CC(=NC1)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 5-[3-hydroxy-5-(1-triisopropylsilanyl-1H-indol-4-yl)-phenylamino]-pyridin-2-ol (taken as 0.126 mmol) in TFA/CH2Cl2 (5 mL/5 mL)) was stirred at 0° C. for 1 h. The resulting mixture was concentrated, and saturated aqueous NaHCO3 was added. The pH was adjusted to around 7 and the mixture was extracted with E...
10.6084/m9.figshare.5104873.v1
null
Silyl protective group
null
c1cccc2[nH]ccc12
c1ccc2[nH]ccc2c1
c1ccccc1.c1ccncc1.c1ccc2[nH]ccc2c1
Other
C(=O)(C(F)(F)F)O.C(Cl)Cl
null
null
CC(C)[Si](C(C)C)(C(C)C)n1ccc2c(-c3cc(O)cc(Nc4ccc(O)nc4)c3)cccc21>C(=O)(C(F)(F)F)O.C(Cl)Cl>Oc1cc(Nc2ccc(O)nc2)cc(-c2cccc3[nH]ccc23)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-da44352d4d494044ba354295353557ff
COc1ccc(COc2cc(Br)cc(Br)c2)cc1.Oc1cccnc1>>COc1ccc(COc2cc(Br)cc(Oc3cccnc3)c2)cc1
BrC=1C=C(C=C(C1)Br)OCC1=CC=C(C=C1)OC.OC=1C=NC=CC1.[H-].[Na+].[OH-].[NH4+]>>BrC=1C=C(OC=2C=NC=CC2)C=C(C1)OCC1=CC=C(C=C1)OC
Br[c:14]1[cH:13][c:11]([Br:12])[cH:10][c:9]([O:8][CH2:7][c:6]2[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:24][cH:23]2)[cH:22]1.[OH:15][c:16]1[cH:17][cH:18][cH:19][n:20][cH:21]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][O:8][c:9]2[cH:10][c:11]([Br:12])[cH:13][c:14]([O:15][c:16]3[cH:17][cH:18][cH:19][n:20][cH:21]3)[cH:22]2)[cH...
COc1ccc(COc2cc(Br)cc(Br)c2)cc1.Oc1cccnc1
COc1ccc(COc2cc(Br)cc(Oc3cccnc3)c2)cc1
null
[Cu]=O
N1=C(C=C(C=C1C)C)C.C(C)(=O)OCC
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
e4ea1e38252bc3b9c5ec04486386725e6570ab3860d45e337a1d131319bbf0fc
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1ccc(COc2cccc(Oc3cccnc3)c2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[OH;D1;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]:[c:11]>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[O;H0;D2;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]:[c:11]):[c:4]:[c:5]
25
[{"value": 25.0, "product": "BrC=1C=C(OC=2C=NC=CC2)C=C(C1)OCC1=CC=C(C=C1)OC", "details": "PERCENTYIELD", "is_desired": false}]
210
CELSIUS
10
MINUTE
A mixture of the 3,5-dibromo-1-p-methoxy-benzyloxybenzene (250 mg, 0.672 mmol) and 3-hydroxypyridine (128 mg, 1.34 mmol) and 96 mg (0.67 mmol) copper oxide in 3 mL of collidine was treated with sodium hydride (27 mg, 0.67 mmol) in a stirred tube. After 10 minutes to allow off-gassing, the tube was sealed and the reacti...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1.c1ccncc1
HBr
[Cu]=O.N1=C(C=C(C=C1C)C)C.C(C)(=O)OCC
210
0.166667
COc1ccc(COc2cc(Br)cc(Br)c2)cc1.Oc1cccnc1>[Cu]=O.N1=C(C=C(C=C1C)C)C.C(C)(=O)OCC>COc1ccc(COc2cc(Br)cc(Oc3cccnc3)c2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9b47ffa855b54e379dbfcda0be4614a0
COc1ccc(COc2cc(Br)cc(Nc3cccnc3)c2)cc1.OB(O)c1ccc2c(c1)OCO2>>COc1ccc(COc2cc(Nc3cccnc3)cc(-c3ccc4c(c3)OCO4)c2)cc1
B(C1=CC2=C(C=C1)OCO2)(O)O.C(C)(C)(C)P(C1=C(C=CC=C1)C1=CC=CC=C1)C(C)(C)C.C([O-])([O-])=O.[Cs+].[Cs+].BrC=1C=C(C=C(C1)OCC1=CC=C(C=C1)OC)NC=1C=NC=CC1>>O1COC2=C1C=CC(=C2)C=2C=C(C=C(C2)OCC2=CC=C(C=C2)OC)NC=2C=NC=CC2
Br[c:20]1[cH:19][c:11]([NH:12][c:13]2[cH:14][cH:15][cH:16][n:17][cH:18]2)[cH:10][c:9]([O:8][CH2:7][c:6]2[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:32][cH:31]2)[cH:30]1.OB(O)[c:21]1[cH:22][cH:23][c:24]2[c:25]([cH:26]1)[O:27][CH2:28][O:29]2>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][O:8][c:9]2[cH:10][c:11]([NH:12][c:13]3[cH:14...
COc1ccc(COc2cc(Br)cc(Nc3cccnc3)c2)cc1.OB(O)c1ccc2c(c1)OCO2
COc1ccc(COc2cc(Nc3cccnc3)cc(-c3ccc4c(c3)OCO4)c2)cc1
null
C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd]
O1CCOCC1
C-C Coupling
Suzuki coupling with boronic acids
4eaac3524feef0fac9270283493ac343cfbd88f66b23f78df9bf06d23e299fd5
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(COc2cc(Nc3cccnc3)cc(-c3ccc4c(c3)OCO4)c2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]-[#8:11]>>[#8:11]-[c:10]:[c:9]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:7]:[c:8]
null
[]
110
CELSIUS
null
null
[3-bromo-5-(4-methoxy-benzyloxy)-phenyl]-pyridin-3-yl-amine (MW=385.26, 193 mg, 0.5 mmol) was placed into a 10 mL microwave reaction tube and placed under a nitrogen atmosphere. 3,4-(Methylenedioxy)phenylboronic acid (MW=165.94, 124 mg, 0.75 mmol), 2-(di-t-butylphosphino)biphenyl (FW 298.41, 15 mg, 0.05 mmol), tris(dib...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccc2c(c1)OCO2
c1ccccc1.c1ccc2c(c1)OCO2
c1ccccc1.c1ccccc1.c1ccncc1.c1ccc2c(c1)OCO2
HBr.B
C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd].O1CCOCC1
110
null
COc1ccc(COc2cc(Br)cc(Nc3cccnc3)c2)cc1.OB(O)c1ccc2c(c1)OCO2>C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd].O1CCOCC1>COc1ccc(COc2cc(Nc3cccnc3)cc(-c3ccc4c(c3)OCO4)c2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-da9dd3df01f34036a31335f47bc8e43d
COc1ccc(COc2cc(Br)cc(Br)c2)cc1.COc1ccc(COc2cc(Br)cc(Nc3ccncc3)c2)cc1.Nc1ccncc1>>Oc1cc(Nc2ccncc2)cc(-c2cccc3[nH]ccc23)c1
BrC=1C=C(C=C(C1)OCC1=CC=C(C=C1)OC)NC1=CC=NC=C1.NC1=CC=NC=C1.BrC1=CC(=CC(=C1)OCC1=CC=C(C=C1)OC)Br.CC1(C2=C(C(=CC=C2)P(C3=CC=CC=C3)C4=CC=CC=C4)OC5=C(C=CC=C51)P(C6=CC=CC=C6)C7=CC=CC=C7)C.CC(C)([O-])C.[Na+]>>N1C=CC2=C(C=CC=C12)C=1C=C(C=C(C1)NC1=CC=NC=C1)O
COc1ccc(COc2c[c:14](Br)[cH:15][c:16](Br)[cH:17]2)cc1.COc1ccc(C[O:1][c:2]2[cH:3][c:4]([NH:5][c:6]3[cH:7][cH:8][n:9][cH:10][cH:11]3)[cH:12][c:13](Br)[cH:23]2)cc1.c1[c:18]([NH2:19])[cH:22][cH:21]n[cH:20]1>>[OH:1][c:2]1[cH:3][c:4]([NH:5][c:6]2[cH:7][cH:8][n:9][cH:10][cH:11]2)[cH:12][c:13](-[c:14]2[cH:15][cH:16][cH:17][c:18...
COc1ccc(COc2cc(Br)cc(Br)c2)cc1.COc1ccc(COc2cc(Br)cc(Nc3ccncc3)c2)cc1.Nc1ccncc1
Oc1cc(Nc2ccncc2)cc(-c2cccc3[nH]ccc23)c1
null
null
O1CCOCC1
C-C Coupling
OtherReaction
c4525d84e43b85cea7e68da85eeb0dbbca68b725fcba237cdd82cb1ed50ccc9c
8153db5c3bfc596b3ddf75a4bcf8f137ac58632dff07224972307439dcfb31bb
c1cc(Nc2ccncc2)cc(-c2cccc3[nH]ccc23)c1
Br-[c;H0;D3;+0:1]1:[c:2]:[c;H0;D3;+0:3](-Br):[cH;D2;+0:4]:c(-O-C-c2:c:c:c(-O-C):c:c:2):c:1.Br-[c;H0;D3;+0:5]1:[c:6]:[c:7]:[c:8]:[c:9](-[O;H0;D2;+0:10]-C-c2:c:c:c(-O-C):c:c:2):[c:11]:1.[NH2;D1;+0:12]-[c;H0;D3;+0:13]1:[cH;D2;+0:14]:[cH;D2;+0:15]:n:[cH;D2;+0:16]:c:1>>[OH;D1;+0:10]-[c:9]1:[c:11]:[c;H0;D3;+0:5](-[c;H0;D3;+0...
null
[]
110
CELSIUS
null
null
[3-Bromo-5-(4-methoxy-benzyloxy)-phenyl]-pyridin-4-yl-amine. A solution of 4-aminopyridine (71 mg, 0.75 mmol), 1,3-dibromo-5-(4-methoxybenzyloxy)benzene (372.0 mg, 1.0 mmol), XantPhos (56 mg, 0.1 mmol), (dibenzylideneacetone)dipalladium (46 mg, 0.05 mmol), and sodium tert-butoxide (192 mg, 2.0 mmol) in dioxane (3 mL) w...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide.Aromatic halide.Ether.Ether.Ether.Ether.Primary amine
Aromatic alcohol
c1ccccc1.c1ccccc1.c1ccccc1.c1ccccc1.c1ccncc1
c1ccccc1.c1ccc2[nH]ccc2c1
c1ccccc1.c1ccncc1.c1ccc2[nH]ccc2c1
HBr
O1CCOCC1
110
null
COc1ccc(COc2cc(Br)cc(Br)c2)cc1.COc1ccc(COc2cc(Br)cc(Nc3ccncc3)c2)cc1.Nc1ccncc1>O1CCOCC1>Oc1cc(Nc2ccncc2)cc(-c2cccc3[nH]ccc23)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d77c24d3aeee4112bb43e55d41702be6
CC1(C)OB(c2cccc3[nH]ccc23)OC1(C)C.CI.COc1ccc(COc2cc(Br)cc(Nc3cccnc3)c2)cc1>>Cn1ccc2c(-c3cc(O)cc(Nc4cccnc4)c3)cccc21.Cn1ccc2c(B3OC(C)(C)C(C)(C)O3)cccc21
BrC=1C=C(C=C(C1)OCC1=CC=C(C=C1)OC)NC=1C=NC=CC1.CC1(OB(OC1(C)C)C1=C2C=CNC2=CC=C1)C.CI>>CN1C=CC2=C(C=CC=C12)B1OC(C(O1)(C)C)(C)C.CN1C=CC2=C(C=CC=C12)C=1C=C(C=C(C1)NC=1C=NC=CC1)O
[nH:2]1[cH:3][cH:4][c:5]2[c:6]([B:31]3[O:32][C:33]([CH3:34])([CH3:35])[C:36]([CH3:37])([CH3:38])[O:39]3)[cH:21][cH:22][cH:23][c:24]12.I[CH3:25].Br[c:41]1[cH:8][c:9]([O:10][CH2:42][c:7]2[cH:20][cH:30][c:29](O[CH3:1])[cH:28][cH:27]2)[cH:11][c:12]([NH:13][c:14]2[cH:15][cH:16][cH:17][n:18][cH:19]2)[cH:40]1>>[CH3:1][n:2]1[c...
CC1(C)OB(c2cccc3[nH]ccc23)OC1(C)C.CI.COc1ccc(COc2cc(Br)cc(Nc3cccnc3)c2)cc1
Cn1ccc2c(-c3cc(O)cc(Nc4cccnc4)c3)cccc21.Cn1ccc2c(B3OC(C)(C)C(C)(C)O3)cccc21
null
null
null
Aromatic Heterocycle Formation
OtherReaction
af7a56d73766cb70c021ce4a40c52bc7e44bdab01e83278398b5aaf001b681c4
24cbf480b9aafe9766583c7f23142629e3af14b057f15f349d5bffd59d6c0b79
c1cc(B2OCCO2)c2cc[nH]c2c1.c1cncc(Nc2cccc(-c3cccc4[nH]ccc34)c2)c1
Br-[c;H0;D3;+0:1]1:[cH;D2;+0:2]:[c;H0;D3;+0:3](-[#7:4]-[c:5]:[c:6]:[#7;a:7]):[c:8]:[c:9](-[O;H0;D2;+0:10]-[CH2;D2;+0:11]-[c;H0;D3;+0:12]2:[cH;D2;+0:13]:[cH;D2;+0:14]:[c;H0;D3;+0:15](-O-[CH3;D1;+0:16]):[c:17]:[cH;D2;+0:18]:2):[cH;D2;+0:19]:1.I-[CH3;D1;+0:20].[#8:21]1-[C:22]-[C:23]-[#8:24]-[B;H0;D3;+0:25]-1-[c;H0;D3;+0:2...
null
[]
null
null
null
null
1-Methyl-4-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-1H-indole was prepared from 4-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-1H-indole and methyl iodide, and was coupled with [3-bromo-5-(4-methoxy-benzyloxy)-phenyl]-pyridin-3-yl-amine in the same manner as described for Example 25. Deprotection was carried ou...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ether.Ether.Boronic ester
Aromatic alcohol.Boronic ester
[B]1OCCO1.c1ccc2[nH]ccc2c1.c1ccccc1.c1ccccc1
c1ccccc1.c1cccc2[nH]ccc12.[B]1OCCO1.c1cccc2[nH]ccc12
c1ccccc1.c1ccncc1.c1cccc2[nH]ccc12.[B]1OCCO1.c1cccc2[nH]ccc12
HBr.I-
null
null
null
CC1(C)OB(c2cccc3[nH]ccc23)OC1(C)C.CI.COc1ccc(COc2cc(Br)cc(Nc3cccnc3)c2)cc1>>Cn1ccc2c(-c3cc(O)cc(Nc4cccnc4)c3)cccc21.Cn1ccc2c(B3OC(C)(C)C(C)(C)O3)cccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d5753192d0224faa86d0e163bf369cc3
COc1cc(Br)cc(Br)c1.Nc1cccnc1>>COc1cc(Br)cc(Nc2cccnc2)c1
BrC1=CC(=CC(=C1)OC)Br.N1=CC(=CC=C1)N.N1C=CC2=C(C=CC=C12)C=1C=C(C=C(C1)OC)NC=1C=NC=CC1>>BrC=1C=C(C=C(C1)OC)NC=1C=NC=CC1
Br[c:8]1[cH:7][c:5]([Br:6])[cH:4][c:3]([O:2][CH3:1])[cH:16]1.[NH2:9][c:10]1[cH:11][cH:12][cH:13][n:14][cH:15]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]([Br:6])[cH:7][c:8]([NH:9][c:10]2[cH:11][cH:12][cH:13][n:14][cH:15]2)[cH:16]1
COc1cc(Br)cc(Br)c1.Nc1cccnc1
COc1cc(Br)cc(Nc2cccnc2)c1
null
null
null
Heteroatom Alkylation and Arylation
N-arylation (Buchwald-Hartwig/Ullmann-Goldberg)
da9dae6a655c4bd18887b692f91621e77027436294d6e1fc7be7295afb364796
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(Nc2cccnc2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]:[c:11]>>[c:8]:[c:7](-[NH;D2;+0:6]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9]:[#7;a:10]:[c:11]
null
[]
null
null
null
null
(3-Bromo-5-methoxy-phenyl)-pyridin-3-yl-amine was prepared from 1,3-dibromo-5-methoxy-benzene and pyridin-3-ylamine as described for Example 36. This material was converted to [3-(1H-indol-4-yl)-5-methoxy-phenyl]-pyridin-3-yl-amine by the method of Example 35. 1H NMR (400 MHz, CDCl3): δ 8.44 (d, J=2.7 Hz, 1H), 8.34 (br...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ccccc1
c1ccccc1
c1ccccc1.c1ccncc1
HBr
null
null
null
COc1cc(Br)cc(Br)c1.Nc1cccnc1>>COc1cc(Br)cc(Nc2cccnc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2bf35fd8a86c4627a60c8cc3d7fda835
COc1ccc(COc2cc(Br)cc(Br)c2)cc1.COc1ccc(COc2cc(Br)cc(C(=O)c3ccc(C)nc3)c2)cc1.Cc1ccc(C#N)cn1>>O=C(c1ccc(CO)nc1)c1cc(O)cc(-c2cccc3[nH]ccc23)c1
Cl.[Li]CCCC.CCCCCC.BrC1=CC(=CC(=C1)OCC1=CC=C(C=C1)OC)Br.BrC=1C=C(C=C(C1)OCC1=CC=C(C=C1)OC)C(=O)C=1C=NC(=CC1)C.CC1=NC=C(C#N)C=C1.[OH-].[Na+]>>OC=1C=C(C=C(C1)C1=C2C=CNC2=CC=C1)C(=O)C=1C=NC(=CC1)CO
COc1ccc(C[O:8][c:21]2[cH:20][c:19](Br)[cH:18][c:17](Br)[cH:25]2)cc1.COc1ccc(C[O:14][c:13]2[cH:12][c:11]([C:2](=[O:1])[c:3]3[cH:4][cH:5][c:6]([CH3:7])[n:9][cH:10]3)[cH:26][c:16](Br)[cH:15]2)cc1.Cc1cc[c:24]([C:23]#[N:22])cn1>>[O:1]=[C:2]([c:3]1[cH:4][cH:5][c:6]([CH2:7][OH:8])[n:9][cH:10]1)[c:11]1[cH:12][c:13]([OH:14])[cH...
COc1ccc(COc2cc(Br)cc(Br)c2)cc1.COc1ccc(COc2cc(Br)cc(C(=O)c3ccc(C)nc3)c2)cc1.Cc1ccc(C#N)cn1
O=C(c1ccc(CO)nc1)c1cc(O)cc(-c2cccc3[nH]ccc23)c1
null
null
CCOCC
Heteroatom Alkylation and Arylation
OtherReaction
e948f15af83dadb9336ecab39fc7779aeb5785da8e178956da39ac376662b95f
7a4ecf18617f425f716e974816027fd0ec9d5b5a6acc9c7a1bd7f5769ccc01b7
O=C(c1cccnc1)c1cccc(-c2cccc3[nH]ccc23)c1
Br-[c;H0;D3;+0:1]1:[c:2]:[c;H0;D3;+0:3](-Br):[c:4]:[c;H0;D3;+0:5](-[O;H0;D2;+0:6]-C-c2:c:c:c(-O-C):c:c:2):[cH;D2;+0:7]:1.Br-[c;H0;D3;+0:8]1:[c:9]:[c:10](-[O;H0;D2;+0:11]-C-c2:c:c:c(-O-C):c:c:2):[c:12]:[c:13](-[C:14]=[O;D1;H0:15]):[c:16]:1.[CH3;D1;+0:17]-[c:18](:[c:19]):[#7;a:20]:[c:21].C-c1:c:c:[c;H0;D3;+0:22](-[C;H0;D...
90
[{"value": 90.0, "product": "OC=1C=C(C=C(C1)C1=C2C=CNC2=CC=C1)C(=O)C=1C=NC(=CC1)CO", "details": "PERCENTYIELD", "is_desired": false}]
-78
CELSIUS
30
MINUTE
[3-Bromo-5-(4-methoxy-benzyloxy)-phenyl]-(6-methyl-pyridin-3-yl)-methanone. A 1.6 M solution of n-BuLi in hexane (1.8 mmol) was added dropwise to a stirred mixture of 1,3-dibromo-5-(4-methoxy-benzyloxy)-benzene (600 mg, 1.6 mmol) in dry ether (6 mL) at −78° C. The resulting solution was stirred at −78° C. for 30 min, a...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide.Aromatic halide.Ether.Ether.Ether.Ether.Nitrile
Primary alcohol.Aromatic alcohol
c1ccccc1.c1ccccc1.c1ccccc1.c1ccccc1.c1ccncc1
c1ccccc1.c1ccc2[nH]ccc2c1
c1ccncc1.c1ccccc1.c1ccc2[nH]ccc2c1
HBr
CCOCC
-78
0.5
COc1ccc(COc2cc(Br)cc(Br)c2)cc1.COc1ccc(COc2cc(Br)cc(C(=O)c3ccc(C)nc3)c2)cc1.Cc1ccc(C#N)cn1>CCOCC>O=C(c1ccc(CO)nc1)c1cc(O)cc(-c2cccc3[nH]ccc23)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7737219f4cf3499a853cb7b39ec051ff
COc1ccc(COc2cc(Br)cc(C(=O)c3ccc(COC(C)=O)nc3)c2)cc1.Cc1ccc(C=O)cn1.O=C(OO)c1cccc(Cl)c1>>O=C(c1ccc(CO)nc1)c1cc(O)cc(-c2cccc3[nH]ccc23)c1
BrC=1C=C(C(=O)C=2C=CC(=NC2)COC(C)=O)C=C(C1)OCC1=CC=C(C=C1)OC.CC1=CC=C(C=N1)C=O.C1=CC(=CC(=C1)Cl)C(=O)OO>>OC=1C=C(C=C(C1)C1=C2C=CNC2=CC=C1)C(=O)C=1C=NC(=CC1)CO
COc1ccc(C[O:14][c:13]2[cH:12][c:11]([C:2](=[O:1])[c:3]3[cH:4][cH:5][c:6]([CH2:7][O:8]C(C)=O)[n:9][cH:10]3)[cH:26][c:16](Br)[cH:15]2)cc1.O=[CH:17][c:25]1[cH:18][cH:19][c:23]([CH3:24])[n:22][cH:21]1.O=C(OO)c1cc[cH:20]c(Cl)c1>>[O:1]=[C:2]([c:3]1[cH:4][cH:5][c:6]([CH2:7][OH:8])[n:9][cH:10]1)[c:11]1[cH:12][c:13]([OH:14])[cH...
COc1ccc(COc2cc(Br)cc(C(=O)c3ccc(COC(C)=O)nc3)c2)cc1.Cc1ccc(C=O)cn1.O=C(OO)c1cccc(Cl)c1
O=C(c1ccc(CO)nc1)c1cc(O)cc(-c2cccc3[nH]ccc23)c1
null
null
C(Cl)Cl
C-C Coupling
OtherReaction
6c8da7ce53fd214ec8dfdab510ef17349306a976a4d3fba782d9e9ab63e3685e
fec724f070bb48acdefa813f4b238dca765a2561241e4f3d05461059818d7190
O=C(c1cccnc1)c1cccc(-c2cccc3[nH]ccc23)c1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[O;H0;D2;+0:4]-C-c2:c:c:c(-O-C):c:c:2):[c:5]:[c:6](-[C:7]=[O;D1;H0:8]):[c:9]:1.C-C(=O)-[O;H0;D2;+0:10]-[C:11]-[c:12]:[#7;a:13].Cl-c1:[cH;D2;+0:14]:c:c:c(-C(=O)-O-O):c:1.O=[CH;D2;+0:15]-[c;H0;D3;+0:16]1:[cH;D2;+0:17]:[cH;D2;+0:18]:[c;H0;D3;+0:19](-[CH3;D1;+0:20]):[n;H0;D2;+0:21]:[cH;D2;+0...
31
[{"value": 31.0, "product": "OC=1C=C(C=C(C1)C1=C2C=CNC2=CC=C1)C(=O)C=1C=NC(=CC1)CO", "details": "PERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
Acetic acid 5-[3-bromo-5-(4-methoxy-benzyloxy)-benzoyl]-pyridin-2-ylmethyl ester. To a stirred solution of 3-bromo-5-(4-methoxy-benzyloxy)-phenyl]-(6-methyl-pyridin-3-yl)-methanone (388 mg, 0.94 mmol) in dry methylene chloride (20 mL) at 0° C. was added dropwise a solution of MCPBA (0.371 mg, 1.50 mmol) in methylene ch...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide.Aldehyde.Ester.Ether.Ether.Peroxide
Primary alcohol.Aromatic alcohol
c1ccccc1.c1ccccc1.c1ccncc1.c1ccccc1
c1ccccc1.c1ccc2[nH]ccc2c1
c1ccncc1.c1ccccc1.c1ccc2[nH]ccc2c1
HCl.Br-
C(Cl)Cl
null
8
COc1ccc(COc2cc(Br)cc(C(=O)c3ccc(COC(C)=O)nc3)c2)cc1.Cc1ccc(C=O)cn1.O=C(OO)c1cccc(Cl)c1>C(Cl)Cl>O=C(c1ccc(CO)nc1)c1cc(O)cc(-c2cccc3[nH]ccc23)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6703728128714fcc8e5ef29e680462c9
CC(C)[Si](C(C)C)(C(C)C)n1ccc2c(B3OC(C)(C)C(C)(C)O3)cccc21.COc1ccc(COc2cc(Br)cc(C(=O)c3ccc(COC(C)=O)nc3)c2)cc1>>O=C(c1ccc(CO)nc1)c1cc(O)cc(-c2cccc3[nH]ccc23)c1
[O-]P(=O)([O-])[O-].[K+].[K+].[K+].BrC=1C=C(C(=O)C=2C=CC(=NC2)COC(C)=O)C=C(C1)OCC1=CC=C(C=C1)OC.COC1=CC=C(COC=2C=C(C(=O)C=3C=CC(=NC3)COC(C)=O)C=C(C2)C2=C3C=CN(C3=CC=C2)[Si](C(C)C)(C(C)C)C(C)C)C=C1.CC1(OB(OC1(C)C)C1=C2C=CN(C2=CC=C1)[Si](C(C)C)(C(C)C)C(C)C)C>>OC=1C=C(C=C(C1)C1=C2C=CNC2=CC=C1)C(=O)C=1C=NC(=CC1)CO
CC(C)[Si](C(C)C)(C(C)C)[n:22]1[c:21]2[cH:20][cH:19][cH:18][c:17](B3OC(C)(C)C(C)(C)O3)[c:25]2[cH:24][cH:23]1.COc1ccc(C[O:14][c:13]2[cH:12][c:11]([C:2](=[O:1])[c:3]3[cH:4][cH:5][c:6]([CH2:7][O:8]C(C)=O)[n:9][cH:10]3)[cH:26][c:16](Br)[cH:15]2)cc1>>[O:1]=[C:2]([c:3]1[cH:4][cH:5][c:6]([CH2:7][OH:8])[n:9][cH:10]1)[c:11]1[cH:...
CC(C)[Si](C(C)C)(C(C)C)n1ccc2c(B3OC(C)(C)C(C)(C)O3)cccc21.COc1ccc(COc2cc(Br)cc(C(=O)c3ccc(COC(C)=O)nc3)c2)cc1
O=C(c1ccc(CO)nc1)c1cc(O)cc(-c2cccc3[nH]ccc23)c1
null
Cl[Pd-](C1=C(C=CC=C1)C1=C(C=CC=C1)N(C)C)P(C1C2CCC(C1)C2)C2C1CCC(C2)C1
O1CCOCC1.C(Cl)Cl
C-C Coupling
OtherReaction
03c0602d335cce017caa249dd9f408403bceda0791224bef598f481caa20bd25
2623277bd6e5f54360592f40b6a823951456d639d0d506a8c2827cddd3033ea0
O=C(c1cccnc1)c1cccc(-c2cccc3[nH]ccc23)c1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[O;H0;D2;+0:4]-C-c2:c:c:c(-O-C):c:c:2):[c:5]:[c:6](-[C:7]=[O;D1;H0:8]):[c:9]:1.C-C(=O)-[O;H0;D2;+0:10]-[C:11]-[c:12]:[#7;a:13].C-C(-C)-[Si](-C(-C)-C)(-C(-C)-C)-[n;H0;D3;+0:14]1:[c:15]:[c:16]:[c:17]2:[c:18]:1:[c:19]:[c:20]:[c:21]:[c;H0;D3;+0:22]:2-B1-O-C(-C)(-C)-C(-C)(-C)-O-1>>[#7;a:13]:[...
null
[]
null
null
null
null
Acetic acid 5-[3-(4-methoxy-benzyloxy)-5-(1-triisopropylsilanyl-1H-indol-4-yl)-benzoyl]-pyridin-2-ylmethyl ester. To the mixture of acetic acid 5-[3-bromo-5-(4-methoxy-benzyloxy)-benzoyl]-pyridin-2-ylmethyl ester (145 mg, 0.308 mmol) and chloro(di-2-norbornylphosphino)(2′dimethylamino-1,1′-biphenyl-2-yl)palladium (II) ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Ether.Ether.Boronic ester.Silyl protective group
Primary alcohol.Aromatic alcohol
c1cccc2[nH]ccc12.B1OCCO1.c1ccccc1.c1ccccc1
c1ccccc1.c1ccc2[nH]ccc2c1
c1ccncc1.c1ccccc1.c1ccc2[nH]ccc2c1
HBr.B
Cl[Pd-](C1=C(C=CC=C1)C1=C(C=CC=C1)N(C)C)P(C1C2CCC(C1)C2)C2C1CCC(C2)C1.O1CCOCC1.C(Cl)Cl
null
null
CC(C)[Si](C(C)C)(C(C)C)n1ccc2c(B3OC(C)(C)C(C)(C)O3)cccc21.COc1ccc(COc2cc(Br)cc(C(=O)c3ccc(COC(C)=O)nc3)c2)cc1>Cl[Pd-](C1=C(C=CC=C1)C1=C(C=CC=C1)N(C)C)P(C1C2CCC(C1)C2)C2C1CCC(C2)C1.O1CCOCC1.C(Cl)Cl>O=C(c1ccc(CO)nc1)c1cc(O)cc(-c2cccc3[nH]ccc23)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ee78f4f15c7742d89b86ba8906c4996d
CC(C)[Si](Oc1cc(C(=O)c2cccnc2)cc(-c2cccc3c2ccn3[Si](C(C)C)(C(C)C)C(C)C)c1)(C(C)C)C(C)C>>CC(O)(c1cccnc1)c1cc(O)cc(-c2cccc3[nH]ccc23)c1
CCCC[N+](CCCC)(CCCC)CCCC.[F-].N1=CC(=CC=C1)C(=O)C1=CC(=CC(=C1)O[Si](C(C)C)(C(C)C)C(C)C)C1=C2C=CN(C2=CC=C1)[Si](C(C)C)(C(C)C)C(C)C.C[Mg]Cl>>OC(C)(C=1C=NC=CC1)C=1C=C(C=C(C1)C1=C2C=CNC2=CC=C1)O
CC(C)[Si](C(C)C)(C(C)C)[O:13][c:12]1[cH:11][c:10]([C:2](=[O:3])[c:4]2[cH:5][cH:6][cH:7][n:8][cH:9]2)[cH:25][c:15](-[c:16]2[cH:17][cH:18][cH:19][c:20]3[n:21]([Si](C(C)C)(C(C)C)C(C)C)[cH:22][cH:23][c:24]23)[cH:14]1>>[CH3:1][C:2]([OH:3])([c:4]1[cH:5][cH:6][cH:7][n:8][cH:9]1)[c:10]1[cH:11][c:12]([OH:13])[cH:14][c:15](-[c:1...
CC(C)[Si](Oc1cc(C(=O)c2cccnc2)cc(-c2cccc3c2ccn3[Si](C(C)C)(C(C)C)C(C)C)c1)(C(C)C)C(C)C
CC(O)(c1cccnc1)c1cc(O)cc(-c2cccc3[nH]ccc23)c1
null
null
[Cl-].[Na+].O.C1CCOC1
Miscellaneous
OtherReaction
7ca7083e374d5c1bb0751ac24fce95f1cc0a06ac813068111afddc4fa2035727
1006a427946ab05af95065220492931e2df745bcea703fed167e9a72cf9ce48d
c1cncc(Cc2cccc(-c3cccc4[nH]ccc34)c2)c1
C-C(-C)-[Si](-C(-C)-C)(-C(-C)-C)-[n;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[c:5]:1:[c:6].C-C(-C)-[Si](-[O;H0;D2;+0:7]-[c:8](:[c:9]):[c:10]:[c:11](-[C;H0;D3;+0:12](=[O;H0;D1;+0:13])-[c:14](:[c:15]):[c:16]:[#7;a:17]:[c:18]):[c:19])(-C(-C)-C)-C(-C)-C>>[C;D1;H3:20]-[C;H0;D4;+0:12](-[OH;D1;+0:13])(-[c:11](:[c:19]):[c:10]:[c:8](-[OH...
39
[{"value": 39.0, "product": "OC(C)(C=1C=NC=CC1)C=1C=C(C=C(C1)C1=C2C=CNC2=CC=C1)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
To pyridin-3-yl-[3-(1-triisopropylsilanyl-1H-indol-4-yl)-5-triisopropylsilanyloxy-phenyl]-methanone (64 mg, 0.102 mmol) in 2 mL of THF was added 2 mL of MeMgCl (1 M in THF) at 0° C. After 30 min TLC indicated the completion of the reaction. Brine was then added to quench the reaction. The aqueous phase was then extract...
10.6084/m9.figshare.5104873.v1
null
Ketone.Silyl protective group.Silyl protective group
Tertiary alcohol.Aromatic alcohol
c1cccc2[nH]ccc12
c1ccc2[nH]ccc2c1
c1ccncc1.c1ccccc1.c1ccc2[nH]ccc2c1
Other
[Cl-].[Na+].O.C1CCOC1
null
0.5
CC(C)[Si](Oc1cc(C(=O)c2cccnc2)cc(-c2cccc3c2ccn3[Si](C(C)C)(C(C)C)C(C)C)c1)(C(C)C)C(C)C>[Cl-].[Na+].O.C1CCOC1>CC(O)(c1cccnc1)c1cc(O)cc(-c2cccc3[nH]ccc23)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1503960581b64c7bacfc5d703c708315
CC(C)(C)[Si](C)(C)Oc1ccc(C(O)c2cccnc2)cc1C12CC3CC(CC(C3)C1)C2>>CC(C)(C)[Si](C)(C)Oc1ccc(C(=O)c2cccnc2)cc1C12CC3CC(CC(C3)C1)C2
C12(CC3CC(CC(C1)C3)C2)C=2C=C(C=CC2O[Si](C)(C)C(C)(C)C)C(O)C=2C=NC=CC2.CC(=O)OI1(C=2C=CC=CC2C(=O)O1)(OC(=O)C)OC(=O)C>>C12(CC3CC(CC(C1)C3)C2)C=2C=C(C=CC2O[Si](C)(C)C(C)(C)C)C(=O)C=2C=NC=CC2
[CH3:1][C:2]([CH3:3])([CH3:4])[Si:5]([CH3:6])([CH3:7])[O:8][c:9]1[cH:10][cH:11][c:12]([CH:13]([OH:14])[c:15]2[cH:16][cH:17][cH:18][n:19][cH:20]2)[cH:21][c:22]1[C:23]12[CH2:24][CH:25]3[CH2:26][CH:27]([CH2:28][CH:29]([CH2:30]3)[CH2:31]1)[CH2:32]2>>[CH3:1][C:2]([CH3:3])([CH3:4])[Si:5]([CH3:6])([CH3:7])[O:8][c:9]1[cH:10][c...
CC(C)(C)[Si](C)(C)Oc1ccc(C(O)c2cccnc2)cc1C12CC3CC(CC(C3)C1)C2
CC(C)(C)[Si](C)(C)Oc1ccc(C(=O)c2cccnc2)cc1C12CC3CC(CC(C3)C1)C2
null
null
CCOCC.C(Cl)Cl
Oxidation
Oxidation or Dehydrogenation of Alcohols to Aldehydes and Ketones
c7c20d2959ac48847b03cc1265962cf99a8ec8a85900c087dabb30077298c66c
767cfd93f5821ebb9e1e72addd9cb404b20b0c821d246ae6b87a5776b74a455b
O=C(c1cccnc1)c1cccc(C23CC4CC(CC(C4)C2)C3)c1
[OH;D1;+0:1]-[CH;D3;+0:2](-[c:3](:[c:4]):[c:5])-[c:6](:[c:7]):[c:8]:[#7;a:9]:[c:10]>>[O;H0;D1;+0:1]=[C;H0;D3;+0:2](-[c:3](:[c:4]):[c:5])-[c:6](:[c:7]):[c:8]:[#7;a:9]:[c:10]
null
[]
null
null
10
MINUTE
[3-Adamantan-1-yl-4-(tert-butyl-dimethyl-silanyloxy)-phenyl]-pyridin-3-yl-methanol (55 mg, 0.112 mmol) was dissolved in methylene chloride. The Dess Martin periodane (0.104 g, 0.224 mmol) was then added to the reaction mixture. The reaction was complete within 10 min and was then diluted with ether. The organic layer w...
10.6084/m9.figshare.5104873.v1
null
Secondary alcohol
Ketone
null
null
c1ccccc1.c1ccncc1.C1C2CC3CC1CC(C2)C3
null
CCOCC.C(Cl)Cl
null
0.166667
CC(C)(C)[Si](C)(C)Oc1ccc(C(O)c2cccnc2)cc1C12CC3CC(CC(C3)C1)C2>CCOCC.C(Cl)Cl>CC(C)(C)[Si](C)(C)Oc1ccc(C(=O)c2cccnc2)cc1C12CC3CC(CC(C3)C1)C2
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-55a5b51c94a14dc0bcea4aac4ff00ba7
COC(=O)c1cc(Br)cc(Br)c1.Nc1cccnc1>>COC(=O)c1cc(Br)cc(Nc2cccnc2)c1
COC(C1=CC(=CC(=C1)Br)Br)=O.N1=CC(=CC=C1)N.COC(C1=CC(=CC(=C1)NC=1C=NC=CC1)C1=C2C=CNC2=CC=C1)=O>>COC(C1=CC(=CC(=C1)NC=1C=NC=CC1)Br)=O
Br[c:10]1[cH:9][c:7]([Br:8])[cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:18]1.[NH2:11][c:12]1[cH:13][cH:14][cH:15][n:16][cH:17]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([Br:8])[cH:9][c:10]([NH:11][c:12]2[cH:13][cH:14][cH:15][n:16][cH:17]2)[cH:18]1
COC(=O)c1cc(Br)cc(Br)c1.Nc1cccnc1
COC(=O)c1cc(Br)cc(Nc2cccnc2)c1
null
null
null
Heteroatom Alkylation and Arylation
N-arylation (Buchwald-Hartwig/Ullmann-Goldberg)
da9dae6a655c4bd18887b692f91621e77027436294d6e1fc7be7295afb364796
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(Nc2cccnc2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]-[C:4](-[#8:5])=[O;D1;H0:6]):[c:7]:[c:8].[NH2;D1;+0:9]-[c:10](:[c:11]):[c:12]:[#7;a:13]:[c:14]>>[#8:5]-[C:4](=[O;D1;H0:6])-[c:3]:[c:2]:[c;H0;D3;+0:1](-[NH;D2;+0:9]-[c:10](:[c:11]):[c:12]:[#7;a:13]:[c:14]):[c:7]:[c:8]
null
[]
null
null
null
null
3-Bromo-5-(pyridin-3-ylamino)-benzoic acid methyl ester was prepared from 3,5-dibromo-benzoic acid methyl ester and pyridin-3-ylamine in low yield as described for Example 36, except that the reaction was run at 130° C. This material was converted to 3-(1H-indol-4-yl)-5-(pyridin-3-ylamino)-benzoic acid methyl ester by ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ccccc1
c1ccccc1
c1ccccc1.c1ccncc1
HBr
null
null
null
COC(=O)c1cc(Br)cc(Br)c1.Nc1cccnc1>>COC(=O)c1cc(Br)cc(Nc2cccnc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5d0e740c926b47bd93f066dc842f030c
N#Cc1cc(Br)cc(Br)c1.Nc1cccnc1>>N#Cc1cc(Br)cc(Nc2cccnc2)c1
BrC=1C=C(C#N)C=C(C1)Br.N1=CC(=CC=C1)N.N1C=CC2=C(C=CC=C12)C=1C=C(C#N)C=C(C1)NC=1C=NC=CC1>>BrC=1C=C(C#N)C=C(C1)NC=1C=NC=CC1
Br[c:8]1[cH:7][c:5]([Br:6])[cH:4][c:3]([C:2]#[N:1])[cH:16]1.[NH2:9][c:10]1[cH:11][cH:12][cH:13][n:14][cH:15]1>>[N:1]#[C:2][c:3]1[cH:4][c:5]([Br:6])[cH:7][c:8]([NH:9][c:10]2[cH:11][cH:12][cH:13][n:14][cH:15]2)[cH:16]1
N#Cc1cc(Br)cc(Br)c1.Nc1cccnc1
N#Cc1cc(Br)cc(Nc2cccnc2)c1
null
null
null
Heteroatom Alkylation and Arylation
N-arylation (Buchwald-Hartwig/Ullmann-Goldberg)
da9dae6a655c4bd18887b692f91621e77027436294d6e1fc7be7295afb364796
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(Nc2cccnc2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9]:[#7;a:10]:[c:11]>>[c:8]:[c:7](-[NH;D2;+0:6]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9]:[#7;a:10]:[c:11]
null
[]
null
null
null
null
3-Bromo-5-(pyridin-3-ylamino)-benzonitrile was prepared from 3,5-dibromobenzonitrile and pyridin-3-ylamine as described for Example 36, except that the reaction was run at 130° C. This material was converted to 3-(1H-indol-4-yl)-5-(pyridin-3-ylamino)-benzonitrile by the method of Example 35. 1H NMR (400 MHz, CDCl3): δ ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ccccc1
c1ccccc1
c1ccccc1.c1ccncc1
HBr
null
null
null
N#Cc1cc(Br)cc(Br)c1.Nc1cccnc1>>N#Cc1cc(Br)cc(Nc2cccnc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-dae9a6a9077749918dfd61060c9a2cdb
COc1ccc(COc2cc(Br)cc(Nc3cccnc3)c2)cc1>>Oc1cc(Br)cc(Nc2cccnc2)c1
BrC=1C=C(C=C(C1)OCC1=CC=C(C=C1)OC)NC=1C=NC=CC1.C1(=CC=CC=C1)SC.FC(C(=O)O)(F)F>>BrC=1C=C(C=C(C1)NC=1C=NC=CC1)O
COc1ccc(C[O:1][c:2]2[cH:3][c:4]([Br:5])[cH:6][c:7]([NH:8][c:9]3[cH:10][cH:11][cH:12][n:13][cH:14]3)[cH:15]2)cc1>>[OH:1][c:2]1[cH:3][c:4]([Br:5])[cH:6][c:7]([NH:8][c:9]2[cH:10][cH:11][cH:12][n:13][cH:14]2)[cH:15]1
COc1ccc(COc2cc(Br)cc(Nc3cccnc3)c2)cc1
Oc1cc(Br)cc(Nc2cccnc2)c1
null
null
O
Reduction
OtherReaction
8a4606e79840bb3d9b3a2e0b7d9ed5648d76ae6cbcc894506db9722ac2624f9a
3165f563067f8d27bb50b0da034e3e854d1ead7f745de7cf575f7ca4cf677789
c1ccc(Nc2cccnc2)cc1
C-O-c1:c:c:c(-C-[O;H0;D2;+0:1]-[c:2](:[c:3]):[c:4]):c:c:1>>[OH;D1;+0:1]-[c:2](:[c:3]):[c:4]
50.2
[{"value": 50.0, "product": "BrC=1C=C(C=C(C1)NC=1C=NC=CC1)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 50.2, "product": "BrC=1C=C(C=C(C1)NC=1C=NC=CC1)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
100
MINUTE
[3-Bromo-5-(4-methoxy-benzyloxy)-phenyl]-pyridin-3-yl-amine (26.7 g, 69.2 mmol) was dissolved in thioanisole (62 mL, 529 mmol). Trifluoroacetic acid (81 mL, 1.06 mol) was added slowly with the temperature held between 20 and 25° C. over a period of 100 min. The solution was left to stand at room temperature for 2 hours...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether
Aromatic alcohol
c1ccccc1
null
c1ccccc1.c1ccncc1
HO-
O
null
1.666667
COc1ccc(COc2cc(Br)cc(Nc3cccnc3)c2)cc1>O>Oc1cc(Br)cc(Nc2cccnc2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c98fbd1f4a384f9ea983660d178fffc7
CC(C)(C)[Si](Cl)(c1ccccc1)c1ccccc1.Oc1cc(Br)cc(Nc2cccnc2)c1>>CC(C)(C)[Si](Oc1cc(Br)cc(Nc2cccnc2)c1)(c1ccccc1)c1ccccc1
BrC=1C=C(C=C(C1)NC=1C=NC=CC1)O.[H-].[Na+].[Si](C1=CC=CC=C1)(C1=CC=CC=C1)(C(C)(C)C)Cl>>BrC=1C=C(C=C(C1)O[Si](C1=CC=CC=C1)(C1=CC=CC=C1)C(C)(C)C)NC=1C=NC=CC1
Cl[Si:5]([C:2]([CH3:1])([CH3:3])[CH3:4])([c:21]1[cH:22][cH:23][cH:24][cH:25][cH:26]1)[c:27]1[cH:28][cH:29][cH:30][cH:31][cH:32]1.[OH:6][c:7]1[cH:8][c:9]([Br:10])[cH:11][c:12]([NH:13][c:14]2[cH:15][cH:16][cH:17][n:18][cH:19]2)[cH:20]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[Si:5]([O:6][c:7]1[cH:8][c:9]([Br:10])[cH:11][c:12]([NH...
CC(C)(C)[Si](Cl)(c1ccccc1)c1ccccc1.Oc1cc(Br)cc(Nc2cccnc2)c1
CC(C)(C)[Si](Oc1cc(Br)cc(Nc2cccnc2)c1)(c1ccccc1)c1ccccc1
null
null
C(C)(C)(C)OC.CN(C)C=O
Protection
Alcohol protection with silyl ethers
b0a79881d208ba0e98fadf827b99c8e154abae20183442d92687b20dcffdaf4c
d57b05ecffa00e68e6b49fce42d0b589b6267b94f85326e13293a0e3abd8a48b
c1ccc([SiH](Oc2cccc(Nc3cccnc3)c2)c2ccccc2)cc1
Cl-[Si;H0;D4;+0:1](-[c:2](:[c:3]):[c:4])(-[c:5](:[c:6]):[c:7])-[C:8](-[C;D1;H3:9])(-[C;D1;H3:10])-[C;D1;H3:11].[OH;D1;+0:12]-[c:13](:[c:14]):[c:15]>>[C;D1;H3:9]-[C:8](-[C;D1;H3:10])(-[C;D1;H3:11])-[Si;H0;D4;+0:1](-[O;H0;D2;+0:12]-[c:13](:[c:14]):[c:15])(-[c:2](:[c:3]):[c:4])-[c:5](:[c:6]):[c:7]
96.1
[{"value": 96.0, "product": "BrC=1C=C(C=C(C1)O[Si](C1=CC=CC=C1)(C1=CC=CC=C1)C(C)(C)C)NC=1C=NC=CC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 96.1, "product": "BrC=1C=C(C=C(C1)O[Si](C1=CC=CC=C1)(C1=CC=CC=C1)C(C)(C)C)NC=1C=NC=CC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
15
MINUTE
3-Bromo-5-(pyridin-3-ylamino)-phenol (11.62 g, 43.83 mmol) was dissolved in DMF (115 mL) under dry argon and cooled to 0° C. Then 60% NaH (1.93 g, 48.21 mmol) was added in small portions over a period of 45 min. Stirring was continued for 15 min, followed by drop wise addition of TBDPS-chloride (11.2 mL, 43.83 mmol). T...
10.6084/m9.figshare.5104873.v1
null
Aromatic alcohol.Silyl protective group
Silyl protective group
null
null
c1ccccc1.c1ccncc1.c1ccccc1.c1ccccc1
HCl
C(C)(C)(C)OC.CN(C)C=O
0
0.25
CC(C)(C)[Si](Cl)(c1ccccc1)c1ccccc1.Oc1cc(Br)cc(Nc2cccnc2)c1>C(C)(C)(C)OC.CN(C)C=O>CC(C)(C)[Si](Oc1cc(Br)cc(Nc2cccnc2)c1)(c1ccccc1)c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ad593bde0fd14ee0b8927e3856b5335d
COc1cc(Br)cc(Br)c1.ClI>>COc1cc(Br)cc(I)c1
BrC1=CC(=CC(=C1)OC)Br.ICl.C(CCC)[Mg]Cl.C(CCC)[Li].CCCCCC>>BrC1=CC(=CC(=C1)OC)I
Br[c:8]1[cH:7][c:5]([Br:6])[cH:4][c:3]([O:2][CH3:1])[cH:10]1.Cl[I:9]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([Br:6])[cH:7][c:8]([I:9])[cH:10]1
COc1cc(Br)cc(Br)c1.ClI
COc1cc(Br)cc(I)c1
null
null
O.C1(=CC=CC=C1)C.C(Cl)Cl
Functional Group Interconversion
OtherReaction
b78ae091f9ea90a571f2e011b77da2eac9952c7b340e2e0185fb0decffadd167
4131cd1655d0ec8ecf7e181a36ab37eb3293d734e38ece0acf0e59405d170401
c1ccccc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].Cl-[I;H0;D1;+0:6]>>[I;H0;D1;+0:6]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
60
[{"value": 60.0, "product": "BrC1=CC(=CC(=C1)OC)I", "details": "PERCENTYIELD", "is_desired": false}, {"value": 60.0, "product": "BrC1=CC(=CC(=C1)OC)I", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-5
CELSIUS
15
MINUTE
A 1.6 M solution of n-butyllithium in hexane (5.65 mL, 9.04 mmol) was dissolved in dry toluene (50 mL) under dry argon and cooled to −5° C. Then a 2M solution of n-butylmagnesium chloride (2.26 mL, 4.52 mmol) was added slowly with the temperature held below 0° C. over a period of 15 min. Stirring was continued for 45 m...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
Aromatic halide
c1ccccc1
c1ccccc1
c1ccccc1
Br-
O.C1(=CC=CC=C1)C.C(Cl)Cl
-5
0.25
COc1cc(Br)cc(Br)c1.ClI>O.C1(=CC=CC=C1)C.C(Cl)Cl>COc1cc(Br)cc(I)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c82d30573024422aae1fd2c8d0f47fec
COc1cc(Br)cc(I)c1>>Oc1cc(Br)cc(I)c1
BrC1=CC(=CC(=C1)OC)I.Br>>BrC=1C=C(C=C(C1)I)O
C[O:1][c:2]1[cH:3][c:4]([Br:5])[cH:6][c:7]([I:8])[cH:9]1>>[OH:1][c:2]1[cH:3][c:4]([Br:5])[cH:6][c:7]([I:8])[cH:9]1
COc1cc(Br)cc(I)c1
Oc1cc(Br)cc(I)c1
null
[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC
C(C)(=O)O
Deprotection
Cleavage of methoxy ethers to alcohols
c5320c7dfa4f544d4900efcae9b3262bf0d5286bcf39c86109232351f35b23d5
26a36596df80ec137b0e8087297418351c93c32819177f680675220622f215d4
c1ccccc1
C-[O;H0;D2;+0:1]-[c:2](:[c:3]):[c:4]>>[OH;D1;+0:1]-[c:2](:[c:3]):[c:4]
352.9
[{"value": 96.0, "product": "BrC=1C=C(C=C(C1)I)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 352.9, "product": "BrC=1C=C(C=C(C1)I)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
DAY
1-Bromo-3-iodo-5-methoxy-benzene (6.29 g, 20.1 mmol) was suspended in a solution of hydrogen bromide in acetic acid (33%, 150 mL). Tetrabutylammonium bromide (0.5 g, 1.55 mmol) was added and the mixture was heated to reflux under vigorous stirring for 2 d. After cooling to room temperature the mixture was extracted wit...
10.6084/m9.figshare.5104873.v1
null
Ether
Aromatic alcohol
null
null
c1ccccc1
Other
[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC.C(C)(=O)O
null
48
COc1cc(Br)cc(I)c1>[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC.C(C)(=O)O>Oc1cc(Br)cc(I)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c5c30b34a447446bb1f71cc9561ce8c5
COc1ccc(CCl)cc1.Oc1cc(Br)cc(I)c1>>COc1ccc(COc2cc(Br)cc(I)c2)cc1
BrC=1C=C(C=C(C1)I)O.C([O-])([O-])=O.[K+].[K+].COC1=CC=C(CCl)C=C1>>BrC1=CC(=CC(=C1)OCC1=CC=C(C=C1)OC)I
Cl[CH2:7][c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:18][cH:17]1.[OH:8][c:9]1[cH:10][c:11]([Br:12])[cH:13][c:14]([I:15])[cH:16]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][O:8][c:9]2[cH:10][c:11]([Br:12])[cH:13][c:14]([I:15])[cH:16]2)[cH:17][cH:18]1
COc1ccc(CCl)cc1.Oc1cc(Br)cc(I)c1
COc1ccc(COc2cc(Br)cc(I)c2)cc1
null
COC1=CC=C(CCl)C=C1
O.C(C)(C)(C)OC.CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
7e1040116e3a4cf0e8ec5cc7865388d9cd0efabce6d320a1c25a36e411018d8b
d5f4610d46ccc0478471c5bc0fb862644eaf764bbc5d93badb39d54f6ec8e0a5
c1ccc(COc2ccccc2)cc1
Cl-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[OH;D1;+0:5]-[c:6](:[c:7]):[c:8]>>[c:7]:[c:6](-[O;H0;D2;+0:5]-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]):[c:8]
77.8
[{"value": 59.0, "product": "BrC1=CC(=CC(=C1)OCC1=CC=C(C=C1)OC)I", "details": "PERCENTYIELD", "is_desired": false}, {"value": 77.8, "product": "BrC1=CC(=CC(=C1)OCC1=CC=C(C=C1)OC)I", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
20
HOUR
3-Bromo-5-iodo-phenol (8.48 g, 28.37 mmol) was dissolved in DMF (50 mL) under dry argon and cooled to 0° C. Then potassium carbonate (3.92 g, 28.37 mmol) was added, followed by drop wise addition of 4-methoxybenzyl chloride (3.7 mL, 27.0 mmol). The mixture was slowly warmed to room temperature and stirred for 20 h. Add...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic alcohol
Ether
null
null
c1ccccc1.c1ccccc1
HCl
COC1=CC=C(CCl)C=C1.O.C(C)(C)(C)OC.CN(C)C=O
0
20
COc1ccc(CCl)cc1.Oc1cc(Br)cc(I)c1>COC1=CC=C(CCl)C=C1.O.C(C)(C)(C)OC.CN(C)C=O>COc1ccc(COc2cc(Br)cc(I)c2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-248392b0c6ba4032a2242aa879019276
CC(C)[Si](C(C)C)(C(C)C)n1ccc2c(B3OC(C)(C)C(C)(C)O3)cccc21.COc1ccc(COc2cc(Br)cc(I)c2)cc1>>COc1ccc(COc2cc(Br)cc(-c3cccc4c3ccn4[Si](C(C)C)(C(C)C)C(C)C)c2)cc1
C([O-])([O-])=O.[Na+].[Na+].CCOC(=O)C.CC1(OB(OC1(C)C)C1=C2C=CN(C2=CC=C1)[Si](C(C)C)(C(C)C)C(C)C)C.BrC1=CC(=CC(=C1)OCC1=CC=C(C=C1)OC)I>>BrC=1C=C(C=C(C1)OCC1=CC=C(C=C1)OC)C1=C2C=CN(C2=CC=C1)[Si](C(C)C)(C(C)C)C(C)C
CC1(C)OB([c:15]2[cH:16][cH:17][cH:18][c:19]3[c:20]2[cH:21][cH:22][n:23]3[Si:24]([CH:25]([CH3:26])[CH3:27])([CH:28]([CH3:29])[CH3:30])[CH:31]([CH3:32])[CH3:33])OC1(C)C.I[c:14]1[cH:13][c:11]([Br:12])[cH:10][c:9]([O:8][CH2:7][c:6]2[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:36][cH:35]2)[cH:34]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]...
CC(C)[Si](C(C)C)(C(C)C)n1ccc2c(B3OC(C)(C)C(C)(C)O3)cccc21.COc1ccc(COc2cc(Br)cc(I)c2)cc1
COc1ccc(COc2cc(Br)cc(-c3cccc4c3ccn4[Si](C(C)C)(C(C)C)C(C)C)c2)cc1
null
null
O.C1(=CC=CC=C1)C.[Cl-].[Na+].O.C(C)O
C-C Coupling
Suzuki coupling with boronic esters
249e9ec88fe1f875d28a2bdea7312c498c739ad3410a41394c8450f214b938e7
b42efb3b6a7742d5af594c6a3031e487327e58e9f8c2f428ee68996c98377910
c1ccc(COc2cccc(-c3cccc4[nH]ccc34)c2)cc1
C-C1(-C)-O-B(-[c;H0;D3;+0:1]2:[c:2]:[c:3]:[c:4]:[c:5]3:[#7;a:6](-[#14:7](-[C:8])(-[C:9])-[C:10]):[c:11]:[c:12]:[c:13]:3:2)-O-C-1(-C)-C.I-[c;H0;D3;+0:14](:[c:15]:[c:16]):[c:17]:[c:18]>>[C:8]-[#14:7](-[C:9])(-[C:10])-[#7;a:6]1:[c:11]:[c:12]:[c:13]2:[c:5]:1:[c:4]:[c:3]:[c:2]:[c;H0;D3;+0:1]:2-[c;H0;D3;+0:14](:[c:15]:[c:16]...
91.3
[{"value": 91.0, "product": "BrC=1C=C(C=C(C1)OCC1=CC=C(C=C1)OC)C1=C2C=CN(C2=CC=C1)[Si](C(C)C)(C(C)C)C(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 91.3, "product": "BrC=1C=C(C=C(C1)OCC1=CC=C(C=C1)OC)C1=C2C=CN(C2=CC=C1)[Si](C(C)C)(C(C)C)C(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false...
90
CELSIUS
14
HOUR
A 1 L flask was charged with 4-(4,4,5,5-tetramethyl-[1,3,2]dioxaborolan-2-yl)-1-triisopropylsilanyl-1H-indole (17.44 g, 43.67 mmol) and 1-Bromo-3-iodo-5-(4-methoxy-benzyloxy)-benzene (18.30 g, 43.67 mmol) in ethanol (180 mL) and toluene (180 mL) under argon. Tetrakis-triphenylphosphin-palladium (1.51 g, 1.31 mmol) was ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic ester
null
B1OCCO1.c1cccc2[nH]ccc12.c1ccccc1
c1ccccc1.c1cccc2[nH]ccc12
c1ccccc1.c1ccccc1.c1cccc2[nH]ccc12
HI.B
O.C1(=CC=CC=C1)C.[Cl-].[Na+].O.C(C)O
90
14
CC(C)[Si](C(C)C)(C(C)C)n1ccc2c(B3OC(C)(C)C(C)(C)O3)cccc21.COc1ccc(COc2cc(Br)cc(I)c2)cc1>O.C1(=CC=CC=C1)C.[Cl-].[Na+].O.C(C)O>COc1ccc(COc2cc(Br)cc(-c3cccc4c3ccn4[Si](C(C)C)(C(C)C)C(C)C)c2)cc1