dataset_id
large_stringclasses
414 values
reaction_id
large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
reactant_smiles
large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ede011a0f2824c2d9586f37aeb9e12dc
CC(O)Cc1cccc(CO[Si](C)(C)C(C)(C)C)c1.[N-]=[N+]=NP(=O)(c1ccccc1)c1ccccc1>>CC(Cc1cccc(CO[Si](C)(C)C(C)(C)C)c1)N=[N+]=[N-]
[Si](C)(C)(C(C)(C)C)OCC=1C=C(C=CC1)CC(C)O.N(=NC(=O)OC(C)C)C(=O)OC(C)C.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(=O)(C1=CC=CC=C1)N=[N+]=[N-]>>N(=[N+]=[N-])C(CC=1C=C(CO[Si](C)(C)C(C)(C)C)C=CC1)C
O[CH:2]([CH3:1])[CH2:3][c:4]1[cH:5][cH:6][cH:7][c:8]([CH2:9][O:10][Si:11]([CH3:12])([CH3:13])[C:14]([CH3:15])([CH3:16])[CH3:17])[cH:18]1.O=P(c1ccccc1)(c1ccccc1)[N:19]=[N+:20]=[N-:21]>>[CH3:1][CH:2]([CH2:3][c:4]1[cH:5][cH:6][cH:7][c:8]([CH2:9][O:10][Si:11]([CH3:12])([CH3:13])[C:14]([CH3:15])([CH3:16])[CH3:17])[cH:18]1)[...
CC(O)Cc1cccc(CO[Si](C)(C)C(C)(C)C)c1.[N-]=[N+]=NP(=O)(c1ccccc1)c1ccccc1
CC(Cc1cccc(CO[Si](C)(C)C(C)(C)C)c1)N=[N+]=[N-]
null
null
ClCCl.C1CCOC1
Heteroatom Alkylation and Arylation
OtherReaction
7ddeb0863eb9d18ad2b86c965fac8ce00b768f5efc2d375573a09ce2ec7becb3
b7a1a21645e453100c6e96f234a0b9438c4e233c7e52a9b671803a56cb864130
c1ccccc1
O-[CH;D3;+0:1](-[C;D1;H3:2])-[C:3]-[c:4].O=P(-[N;H0;D2;+0:5]=[#7;+:6]=[N;-;D1;H0:7])(-c1:c:c:c:c:c:1)-c1:c:c:c:c:c:1>>[C;D1;H3:2]-[CH;D3;+0:1](-[C:3]-[c:4])-[N;H0;D2;+0:5]=[#7;+:6]=[N;-;D1;H0:7]
null
[]
0
CELSIUS
15
MINUTE
To a stirring solution of 1-[3-(tert-butyldimethylsilyloxymethyl)-phenyl]-propan-2-ol (130 mg, 0.46 mmol) in THF (1.5 mL) under nitrogen at 0° C. was added diisopropyl azodicarboxylate (140 mg, 0.7 mmol), triphenylphosphine (180 mg, 0.7 mmol), and diphenylphosphoryl azide (190 mg, 0.7 mmol) and the mixture was stirred ...
10.6084/m9.figshare.5104873.v1
null
Azide.Secondary alcohol
Azide
c1ccccc1.c1ccccc1
null
c1ccccc1
HO-
ClCCl.C1CCOC1
0
0.25
CC(O)Cc1cccc(CO[Si](C)(C)C(C)(C)C)c1.[N-]=[N+]=NP(=O)(c1ccccc1)c1ccccc1>ClCCl.C1CCOC1>CC(Cc1cccc(CO[Si](C)(C)C(C)(C)C)c1)N=[N+]=[N-]
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c4a63c857a0149238c90e001ea0ed467
CCOC(=O)CCC1CN(c2ccnc(NCCc3ccccc3)n2)c2nc(-c3ccccc3)cc(=O)n2C1>>O=C(O)CCC1CN(c2ccnc(NCCc3ccccc3)n2)c2nc(-c3ccccc3)cc(=O)n2C1
C(C)OC(CCC1CN(C=2N(C1)C(C=C(N2)C2=CC=CC=C2)=O)C2=NC(=NC=C2)NCCC2=CC=CC=C2)=O.[OH-].[Li+]>>O=C1C=C(N=C2N1CC(CN2C2=NC(=NC=C2)NCCC2=CC=CC=C2)CCC(=O)O)C2=CC=CC=C2
CC[O:3][C:2](=[O:1])[CH2:4][CH2:5][CH:6]1[CH2:7][N:8]([c:9]2[cH:10][cH:11][n:12][c:13]([NH:14][CH2:15][CH2:16][c:17]3[cH:18][cH:19][cH:20][cH:21][cH:22]3)[n:23]2)[c:24]2[n:25][c:26](-[c:27]3[cH:28][cH:29][cH:30][cH:31][cH:32]3)[cH:33][c:34](=[O:35])[n:36]2[CH2:37]1>>[O:1]=[C:2]([OH:3])[CH2:4][CH2:5][CH:6]1[CH2:7][N:8](...
CCOC(=O)CCC1CN(c2ccnc(NCCc3ccccc3)n2)c2nc(-c3ccccc3)cc(=O)n2C1
O=C(O)CCC1CN(c2ccnc(NCCc3ccccc3)n2)c2nc(-c3ccccc3)cc(=O)n2C1
null
null
O1CCCC1
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=c1cc(-c2ccccc2)nc2n1CCCN2c1ccnc(NCCc2ccccc2)n1
C-C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
null
[]
null
null
null
null
A solution of 3-[6-oxo-1-(2-phenethylamino-pyrimidin-4-yl)-8-phenyl-1,3,4,6-tetrahydro-2H-pyrimido[1,2-a]pyrimidin-3-yl]-propionic acid ethyl ester (240 mg, 0.46 mmol), 10% aqueous lithium hydroxide (0.2 mL), and tetrahydrofuran (5 mL) was heated to 50° C. Reaction partitioned between dichloromethane (50 mL) and 5% sod...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1cncnc1.c1ccccc1.c1ccn2c(n1)NC[CH]C2.c1ccccc1
Other
O1CCCC1
null
null
CCOC(=O)CCC1CN(c2ccnc(NCCc3ccccc3)n2)c2nc(-c3ccccc3)cc(=O)n2C1>O1CCCC1>O=C(O)CCC1CN(c2ccnc(NCCc3ccccc3)n2)c2nc(-c3ccccc3)cc(=O)n2C1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d242b8ffa3834548bc2828bbe0993657
O=C(NCCC1CN(c2ccnc(NCCc3ccccc3)n2)c2nc(-c3ccccc3)cc(=O)n2C1)OCc1ccccc1>>NCCC1CN(c2ccnc(NCCc3ccccc3)n2)c2nc(-c3ccccc3)cc(=O)n2C1
C(C1=CC=CC=C1)OC(NCCC1CN(C=2N(C1)C(C=C(N2)C2=CC=CC=C2)=O)C2=NC(=NC=C2)NCCC2=CC=CC=C2)=O.ClCCl.[H][H]>>NCCC1CN(C=2N(C(C=C(N2)C2=CC=CC=C2)=O)C1)C1=NC(=NC=C1)NCCC1=CC=CC=C1
O=C(OCc1ccccc1)[NH:1][CH2:2][CH2:3][CH:4]1[CH2:5][N:6]([c:7]2[cH:8][cH:9][n:10][c:11]([NH:12][CH2:13][CH2:14][c:15]3[cH:16][cH:17][cH:18][cH:19][cH:20]3)[n:21]2)[c:22]2[n:23][c:24](-[c:25]3[cH:26][cH:27][cH:28][cH:29][cH:30]3)[cH:31][c:32](=[O:33])[n:34]2[CH2:35]1>>[NH2:1][CH2:2][CH2:3][CH:4]1[CH2:5][N:6]([c:7]2[cH:8][...
O=C(NCCC1CN(c2ccnc(NCCc3ccccc3)n2)c2nc(-c3ccccc3)cc(=O)n2C1)OCc1ccccc1
NCCC1CN(c2ccnc(NCCc3ccccc3)n2)c2nc(-c3ccccc3)cc(=O)n2C1
null
[Pd]
CO
Reduction
Hydrogenolysis of amides/imides/carbamates
087b6600ba91d3df931fe6979f2445c192cbfd59e04fd2d8a10f7c7573ac669f
4e549866ec1acadec4c84aaf8495992a28ec78d8ea5ef1b9f44dd843b0dcb7d4
O=c1cc(-c2ccccc2)nc2n1CCCN2c1ccnc(NCCc2ccccc2)n1
O=C(-O-C-c1:c:c:c:c:c:1)-[NH;D2;+0:1]-[C:2]-[C:3]>>[C:3]-[C:2]-[NH2;D1;+0:1]
null
[]
null
null
null
null
A solution of {2-[6-Oxo-1-(2-phenethylamino-pyrimidin-4-yl)-8-phenyl-1,3,4,6-tetrahydro-2H-pyrimido[1,2-a]pyrimidin-3-yl]-ethyl}-carbamic acid benzyl ester (100 mg, 0.17 mmol), dichloromethane (5 mL) and methanol (15 mL) was added 10% palladium on carbon (5 mg) and stirred at room temperature over an atmosphere of hydr...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether
Primary amine
c1ccccc1
null
c1cncnc1.c1ccccc1.c1ccn2c(n1)NC[CH]C2.c1ccccc1
HO-
[Pd].CO
null
null
O=C(NCCC1CN(c2ccnc(NCCc3ccccc3)n2)c2nc(-c3ccccc3)cc(=O)n2C1)OCc1ccccc1>[Pd].CO>NCCC1CN(c2ccnc(NCCc3ccccc3)n2)c2nc(-c3ccccc3)cc(=O)n2C1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-13259bf123d54673ac4b4e67de5cd963
CC(C)=O.NCCC1CN(c2ccnc(NCCc3ccccc3)n2)c2nc(-c3ccccc3)cc(=O)n2C1>>CC(C)NCCC1CN(c2ccnc(NCCc3ccccc3)n2)c2nc(-c3ccccc3)cc(=O)n2C1
C(C)(=O)O[BH-](OC(C)=O)OC(C)=O.[Na+].NCCC1CN(C=2N(C(C=C(N2)C2=CC=CC=C2)=O)C1)C1=NC(=NC=C1)NCCC1=CC=CC=C1.CC(=O)C.ClCCl>>C(C)(C)NCCC1CN(C=2N(C(C=C(N2)C2=CC=CC=C2)=O)C1)C1=NC(=NC=C1)NCCC1=CC=CC=C1
O=[C:2]([CH3:1])[CH3:3].[NH2:4][CH2:5][CH2:6][CH:7]1[CH2:8][N:9]([c:10]2[cH:11][cH:12][n:13][c:14]([NH:15][CH2:16][CH2:17][c:18]3[cH:19][cH:20][cH:21][cH:22][cH:23]3)[n:24]2)[c:25]2[n:26][c:27](-[c:28]3[cH:29][cH:30][cH:31][cH:32][cH:33]3)[cH:34][c:35](=[O:36])[n:37]2[CH2:38]1>>[CH3:1][CH:2]([CH3:3])[NH:4][CH2:5][CH2:6...
CC(C)=O.NCCC1CN(c2ccnc(NCCc3ccccc3)n2)c2nc(-c3ccccc3)cc(=O)n2C1
CC(C)NCCC1CN(c2ccnc(NCCc3ccccc3)n2)c2nc(-c3ccccc3)cc(=O)n2C1
null
null
CO
Heteroatom Alkylation and Arylation
Reductive amination with ketone
4940e8ed9a0db9bde699fdcdc3aff2cff0409c19478aa0ed1acfd98213338adf
07faf85ffe990e88a1de7fd04a339bf226f78d8bfae9712ea59eebd76bb54b9f
O=c1cc(-c2ccccc2)nc2n1CCCN2c1ccnc(NCCc2ccccc2)n1
O=[C;H0;D3;+0:1](-[C;D1;H3:2])-[C;D1;H3:3].[C:4]-[C:5]-[NH2;D1;+0:6]>>[C:4]-[C:5]-[NH;D2;+0:6]-[CH;D3;+0:1](-[C;D1;H3:2])-[C;D1;H3:3]
null
[]
null
null
2
HOUR
To a solution of 7-(2-Amino-ethyl)-9-(2-phenethylamino-pyrimidin-4-yl)-2-phenyl-6,7,8,9-tetrahydro-pyrimido[1,2-a]pyrimidin-4-one (70 mg, 0.15 mmol), acetone (0.02 mL), dichloromethane (0.5 mL) and methanol (0.5 mL) was added sodium triacetoxyborohydride (38 mg, 0.18 mmol) Reaction stirred for 2 h at room temperature. ...
10.6084/m9.figshare.5104873.v1
null
Ketone.Primary amine
Secondary amine
null
null
c1cncnc1.c1ccccc1.c1ccn2c(n1)NC[CH]C2.c1ccccc1
Other
CO
null
2
CC(C)=O.NCCC1CN(c2ccnc(NCCc3ccccc3)n2)c2nc(-c3ccccc3)cc(=O)n2C1>CO>CC(C)NCCC1CN(c2ccnc(NCCc3ccccc3)n2)c2nc(-c3ccccc3)cc(=O)n2C1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-39cb08f716ea46fc9d7265a15ce12e7a
CI.Nc1nc(-c2ccccc2)cc(=O)[nH]1>>Cn1c(N)nc(-c2ccccc2)cc1=O
CI.[OH-].[K+].CI.NC1=NC(=CC(N1)=O)C1=CC=CC=C1>>NC1=NC(=CC(N1C)=O)C1=CC=CC=C1
I[CH3:1].[nH:2]1[c:3]([NH2:4])[n:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][cH:11][cH:12]2)[cH:13][c:14]1=[O:15]>>[CH3:1][n:2]1[c:3]([NH2:4])[n:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][cH:11][cH:12]2)[cH:13][c:14]1=[O:15]
CI.Nc1nc(-c2ccccc2)cc(=O)[nH]1
Cn1c(N)nc(-c2ccccc2)cc1=O
null
null
CCO
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
8b8b604c36c54bca847ea1bd1b7840d48f065047e5c951a27f860631728323c9
7a358c636daddc97c1fb4c29f378044d7eac3f01815d9966e599841f642d631a
O=c1cc(-c2ccccc2)nc[nH]1
I-[CH3;D1;+0:1].[N;D1;H2:2]-[c:3]1:[#7;a:4]:[c:5]:[c:6]:[c:7](=[O;D1;H0:8]):[nH;D2;+0:9]:1>>[CH3;D1;+0:1]-[n;H0;D3;+0:9]1:[c:7](=[O;D1;H0:8]):[c:6]:[c:5]:[#7;a:4]:[c:3]:1-[N;D1;H2:2]
null
[]
null
null
3
DAY
A mixture of KOH (1.22 g, 22 mmol), MeI (6.85 g, 48 mmol), and 2-amino-6-phenyl-3H-pyrimidin-4-one (2.62 g, 14 mmol) in EtOH (130 mL) was stirred at room temperature in a stoppered 250 mL roundbottom flask for 3 days. An additional 6.85 g (48 mmol) MeI was added and stirring was continued for 1 day. The solvent was rem...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ccncn1
c1cncnc1
c1cncnc1.c1ccccc1
HI
CCO
null
72
CI.Nc1nc(-c2ccccc2)cc(=O)[nH]1>CCO>Cn1c(N)nc(-c2ccccc2)cc1=O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c36ac95a2c8f4a28bbcb4b4b9223578e
CC(N)Cc1cccc(CO)c1.Cn1c(Nc2ccnc(S(C)=O)n2)nc(-c2ccccc2)cc1=O>>CC(Cc1cccc(CO)c1)Nc1nccc(Nc2nc(-c3ccccc3)cc(=O)n2C)n1
NC(CC=1C=C(C=CC1)CO)C.CS(=O)C1=NC=CC(=N1)NC1=NC(=CC(N1C)=O)C1=CC=CC=C1.CCOC(=O)C>>OCC=1C=C(C=CC1)CC(C)NC1=NC=CC(=N1)NC1=NC(=CC(N1C)=O)C1=CC=CC=C1
[CH3:1][CH:2]([CH2:3][c:4]1[cH:5][cH:6][cH:7][c:8]([CH2:9][OH:10])[cH:11]1)[NH2:12].CS(=O)[c:13]1[n:14][cH:15][cH:16][c:17]([NH:18][c:19]2[n:20][c:21](-[c:22]3[cH:23][cH:24][cH:25][cH:26][cH:27]3)[cH:28][c:29](=[O:30])[n:31]2[CH3:32])[n:33]1>>[CH3:1][CH:2]([CH2:3][c:4]1[cH:5][cH:6][cH:7][c:8]([CH2:9][OH:10])[cH:11]1)[N...
CC(N)Cc1cccc(CO)c1.Cn1c(Nc2ccnc(S(C)=O)n2)nc(-c2ccccc2)cc1=O
CC(Cc1cccc(CO)c1)Nc1nccc(Nc2nc(-c3ccccc3)cc(=O)n2C)n1
null
null
CN1CCCC1=O
Heteroatom Alkylation and Arylation
OtherReaction
ac54b6a0f3a60d8937c1d499ecd10bb03cfe7d9c83e017605df8cdfb870cd022
5d96541e7662f23805fb9b1f27c86ee9e32f55f6d2b692c46751dd2fe7aa65a5
O=c1cc(-c2ccccc2)nc(Nc2ccnc(NCCc3ccccc3)n2)[nH]1
C-S(=O)-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[#7;a:4]:[c:5].[C:6]-[C:7](-[C;D1;H3:8])-[NH2;D1;+0:9]>>[C:6]-[C:7](-[C;D1;H3:8])-[NH;D2;+0:9]-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[#7;a:4]:[c:5]
null
[]
100
CELSIUS
null
null
A mixture of [3-(2-amino-propyl) -phenyl]-methanol (300 mg, 1.8 mmol) and 2-(2-methanesulfinyl-pyrimidin-4-ylamino) -3-methyl-6-phenyl-3H-pyrimidin-4-one (300 mg, 0.9 mmol) in NMP (8 mL) was heated to 100° C. for 16 h. The reaction was cooled to room temperature and EtOAc was added. The mixture was then washed with H2O...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfoxide
Secondary amine
c1cncnc1
c1cncnc1
c1ccccc1.c1cncnc1.c1cncnc1.c1ccccc1
Other
CN1CCCC1=O
100
null
CC(N)Cc1cccc(CO)c1.Cn1c(Nc2ccnc(S(C)=O)n2)nc(-c2ccccc2)cc1=O>CN1CCCC1=O>CC(Cc1cccc(CO)c1)Nc1nccc(Nc2nc(-c3ccccc3)cc(=O)n2C)n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3548fe0a340042d59fd4d020a5eaab90
C=CC(=O)OCC.CC(NC(=O)OC(C)(C)C)c1ccc(Br)cc1>>CCOC(=O)C=Cc1ccc(C(C)NC(=O)OC(C)(C)C)cc1
C(C=C)(=O)OCC.C(C)(C)(C)P(C(C)(C)C)C(C)(C)C.C(C)(C)(C)OC(NC(C)C1=CC=C(C=C1)Br)=O.CN(C1CCCCC1)C1CCCCC1>>C(C)OC(C=CC1=CC=C(C=C1)C(C)NC(=O)OC(C)(C)C)=O
[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]=[CH2:7].Br[c:8]1[cH:9][cH:10][c:11]([CH:12]([CH3:13])[NH:14][C:15](=[O:16])[O:17][C:18]([CH3:19])([CH3:20])[CH3:21])[cH:22][cH:23]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]=[CH:7][c:8]1[cH:9][cH:10][c:11]([CH:12]([CH3:13])[NH:14][C:15](=[O:16])[O:17][C:18]([CH3:19])([CH3:20])[CH3:2...
C=CC(=O)OCC.CC(NC(=O)OC(C)(C)C)c1ccc(Br)cc1
CCOC(=O)C=Cc1ccc(C(C)NC(=O)OC(C)(C)C)cc1
null
C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd]
O1CCOCC1.O
C-C Coupling
Heck terminal vinyl
55becfded1a3842d5a03bbf3e1610411c659aff0806930400c4db2ef61f9c87f
4b186811a4930853b446d93d9faa39b267bddb9ce0b8021bda5c5a3b2bc69f0b
c1ccccc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[C:6]-[#8:7]-[C:8](=[O;D1;H0:9])-[C:10]=[CH2;D1;+0:11]>>[C:6]-[#8:7]-[C:8](=[O;D1;H0:9])-[C:10]=[CH;D2;+0:11]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
null
[]
80
CELSIUS
null
null
To a mixture of [1-(4-bromo-phenyl)-ethyl]-carbamic acid tert-butyl ester (3.0 g, 10 mmol), tris(dibenzylideneacetone)dipalladium (0.55 g, 0.6 mmol), and N -methyldicyclohexylamine (2.1 mL, 10 mmol) was purged nitrogen followed by the addition of 1,4-dioxane (20 mL) and tri-tert-butylphospine (0.24 g, 1.2 mmol). The mi...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Vinyl
null
c1ccccc1
c1ccccc1
c1ccccc1
HBr
C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd].O1CCOCC1.O
80
null
C=CC(=O)OCC.CC(NC(=O)OC(C)(C)C)c1ccc(Br)cc1>C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd].O1CCOCC1.O>CCOC(=O)C=Cc1ccc(C(C)NC(=O)OC(C)(C)C)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-03202a9215ad4d28aa44793bae1ae8ea
CCOC(=O)C=Cc1ccc(C(C)NC(=O)OC(C)(C)C)cc1>>CCOC(=O)CCc1ccc(C(C)NC(=O)OC(C)(C)C)cc1
C(C)OC(C=CC1=CC=C(C=C1)C(C)NC(=O)OC(C)(C)C)=O>>C(C)OC(CCC1=CC=C(C=C1)C(C)NC(=O)OC(C)(C)C)=O
[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]=[CH:7][c:8]1[cH:9][cH:10][c:11]([CH:12]([CH3:13])[NH:14][C:15](=[O:16])[O:17][C:18]([CH3:19])([CH3:20])[CH3:21])[cH:22][cH:23]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][CH2:7][c:8]1[cH:9][cH:10][c:11]([CH:12]([CH3:13])[NH:14][C:15](=[O:16])[O:17][C:18]([CH3:19])([CH3:20])[CH3:21])...
CCOC(=O)C=Cc1ccc(C(C)NC(=O)OC(C)(C)C)cc1
CCOC(=O)CCc1ccc(C(C)NC(=O)OC(C)(C)C)cc1
null
[OH-].[OH-].[Pd+2]
C(C)O
Reduction
Hydrogenation (double to single)
c04c38f95d7b746e5bdb99c368a7a33956c97b95b54c7ad89be2a85526386ec9
9a50abf8d2e4cd9195d7a0cadbe97483a261a81cf70b653cfddd5ecf76d383a6
c1ccccc1
[C:1]-[#8:2]-[C:3](=[O;D1;H0:4])-[CH;D2;+0:5]=[CH;D2;+0:6]-[c:7](:[c:8]):[c:9]>>[C:1]-[#8:2]-[C:3](=[O;D1;H0:4])-[CH2;D2;+0:5]-[CH2;D2;+0:6]-[c:7](:[c:8]):[c:9]
null
[]
null
null
null
null
Through a mixture of 3-[4-(1-tert-butoxycarbonylamino-ethyl)-phenyl]-acrylic acid ethyl ester (0.22 g, 0.69 mmol) and palladium hydroxide on carbon (100 mg) in ethanol (10 mL) was bubbled hydrogen through a balloon for 17 h. The mixture was filtered through celite and concentrated to afford an off-white solid. M+1=322....
10.6084/m9.figshare.5104873.v1
null
Ester
Ester
null
null
c1ccccc1
null
[OH-].[OH-].[Pd+2].C(C)O
null
null
CCOC(=O)C=Cc1ccc(C(C)NC(=O)OC(C)(C)C)cc1>[OH-].[OH-].[Pd+2].C(C)O>CCOC(=O)CCc1ccc(C(C)NC(=O)OC(C)(C)C)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1aecb3e8b14b42bcb46ebaf03ae1008f
CC(NC(=O)OC(C)(C)C)c1ccc(CCNC(=O)OCc2ccccc2)cc1>>CC(NC(=O)OC(C)(C)C)c1ccc(CCN)cc1
C(C)(C)(C)OC(NC(C)C1=CC=C(C=C1)CCNC(=O)OCC1=CC=CC=C1)=O.C1=CCC=CC1.CO>>C(C)(C)(C)OC(NC(C)C1=CC=C(C=C1)CCN)=O
O=C(OCc1ccccc1)[NH:17][CH2:16][CH2:15][c:14]1[cH:13][cH:12][c:11]([CH:2]([CH3:1])[NH:3][C:4](=[O:5])[O:6][C:7]([CH3:8])([CH3:9])[CH3:10])[cH:19][cH:18]1>>[CH3:1][CH:2]([NH:3][C:4](=[O:5])[O:6][C:7]([CH3:8])([CH3:9])[CH3:10])[c:11]1[cH:12][cH:13][c:14]([CH2:15][CH2:16][NH2:17])[cH:18][cH:19]1
CC(NC(=O)OC(C)(C)C)c1ccc(CCNC(=O)OCc2ccccc2)cc1
CC(NC(=O)OC(C)(C)C)c1ccc(CCN)cc1
null
[Pd]
C(C)O
Reduction
Hydrogenolysis of amides/imides/carbamates
087b6600ba91d3df931fe6979f2445c192cbfd59e04fd2d8a10f7c7573ac669f
4e549866ec1acadec4c84aaf8495992a28ec78d8ea5ef1b9f44dd843b0dcb7d4
c1ccccc1
O=C(-O-C-c1:c:c:c:c:c:1)-[NH;D2;+0:1]-[C:2]-[C:3]>>[C:3]-[C:2]-[NH2;D1;+0:1]
null
[]
null
null
null
null
The mixture of {1-[4-(2-benzyloxycarbonylamino-ethyl)-phenyl]-ethyl}carbamic acid tert-butyl ester (0.80 g, 2.0 mmol), 1,4-cyclohexadiene (0.96 mL, 10 mmol) and palladium on carbon (100 mg) in ethanol (20 mL)-methanol (5 mL) was heated to reflux for 2 h and brought to room temperature. The mixture was filtered through ...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether
Primary amine
c1ccccc1
null
c1ccccc1
HO-
[Pd].C(C)O
null
null
CC(NC(=O)OC(C)(C)C)c1ccc(CCNC(=O)OCc2ccccc2)cc1>[Pd].C(C)O>CC(NC(=O)OC(C)(C)C)c1ccc(CCN)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-da297c3cf29b4412bf3fcc93f12a5406
CC(NC(=O)OC(C)(C)C)c1ccc(CCN)cc1.CS(=O)(=O)c1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1>>CC(NC(=O)OC(C)(C)C)c1ccc(CCNc2nccc(N3CCC(=O)N4CC=C(c5ccccc5)N=C43)n2)cc1
CS(=O)(=O)C1=NC=CC(=N1)N1C=2N(C(CC1)=O)CC=C(N2)C2=CC=CC=C2.C(C)(C)(C)OC(NC(C)C1=CC=C(C=C1)CCN)=O.O1CCOCC1>>C(C)(C)(C)OC(NC(C)C1=CC=C(C=C1)CCNC1=NC=CC(=N1)N1C=2N(C(CC1)=O)CC=C(N2)C2=CC=CC=C2)=O
[CH3:1][CH:2]([NH:3][C:4](=[O:5])[O:6][C:7]([CH3:8])([CH3:9])[CH3:10])[c:11]1[cH:12][cH:13][c:14]([CH2:15][CH2:16][NH2:17])[cH:41][cH:42]1.CS(=O)(=O)[c:18]1[n:19][cH:20][cH:21][c:22]([N:23]2[CH2:24][CH2:25][C:26](=[O:27])[N:28]3[CH2:29][CH:30]=[C:31]([c:32]4[cH:33][cH:34][cH:35][cH:36][cH:37]4)[N:38]=[C:39]23)[n:40]1>>...
CC(NC(=O)OC(C)(C)C)c1ccc(CCN)cc1.CS(=O)(=O)c1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
CC(NC(=O)OC(C)(C)C)c1ccc(CCNc2nccc(N3CCC(=O)N4CC=C(c5ccccc5)N=C43)n2)cc1
null
null
CN1C(CCC1)=O
Heteroatom Alkylation and Arylation
OtherReaction
289adcacbe89f1503fb3c9d1b660927aaeb421d7b5520077738f22dce3010144
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=C1CCN(c2ccnc(NCCc3ccccc3)n2)C2=NC(c3ccccc3)=CCN12
C-S(=O)(=O)-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[#7;a:4]:[c:5].[C:6]-[C:7]-[NH2;D1;+0:8]>>[C:6]-[C:7]-[NH;D2;+0:8]-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[#7;a:4]:[c:5]
null
[]
null
null
null
null
The mixture of 1-(2-methanesulfonyl-pyrimidin-4-yl)-8-phenyl-1,2,3,6-tetrahydro -pyrimido[1,2-a]pyrimidin-4-one (0.20 g, 053 mmol) and {1-[4-(2-amino -ethyl)-phenyl]-ethyl}-carbamic acid tert-butyl ester (0.304 g, 0.79 mmol) in 1:1 dioxane: 1-methyl -2-pyrrolidinone (6 mL) was heated to 100° C. for 17 h. The mixture wa...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cncnc1
c1cncnc1
c1ccccc1.c1cncnc1.C1=CN=C2[NH]CCCN2C1.c1ccccc1
HO-
CN1C(CCC1)=O
null
null
CC(NC(=O)OC(C)(C)C)c1ccc(CCN)cc1.CS(=O)(=O)c1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1>CN1C(CCC1)=O>CC(NC(=O)OC(C)(C)C)c1ccc(CCNc2nccc(N3CCC(=O)N4CC=C(c5ccccc5)N=C43)n2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ef3eca606b604be5a9ee6c58e663f477
CC(N)Cc1ccc(CO)cc1.CS(=O)(=O)c1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1>>CC(Cc1ccc(CO)cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
CS(=O)(=O)C1=NC=CC(=N1)N1C=2N(C(CC1)=O)CC=C(N2)C2=CC=CC=C2.NC(CC1=CC=C(C=C1)CO)C.O1CCOCC1>>OCC1=CC=C(C=C1)CC(C)NC1=NC=CC(=N1)N1C=2N(C(CC1)=O)CC=C(N2)C2=CC=CC=C2
[CH3:1][CH:2]([CH2:3][c:4]1[cH:5][cH:6][c:7]([CH2:8][OH:9])[cH:10][cH:11]1)[NH2:12].CS(=O)(=O)[c:13]1[n:14][cH:15][cH:16][c:17]([N:18]2[CH2:19][CH2:20][C:21](=[O:22])[N:23]3[CH2:24][CH:25]=[C:26]([c:27]4[cH:28][cH:29][cH:30][cH:31][cH:32]4)[N:33]=[C:34]23)[n:35]1>>[CH3:1][CH:2]([CH2:3][c:4]1[cH:5][cH:6][c:7]([CH2:8][OH...
CC(N)Cc1ccc(CO)cc1.CS(=O)(=O)c1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
CC(Cc1ccc(CO)cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
null
null
CN1C(CCC1)=O
Heteroatom Alkylation and Arylation
OtherReaction
289adcacbe89f1503fb3c9d1b660927aaeb421d7b5520077738f22dce3010144
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=C1CCN(c2ccnc(NCCc3ccccc3)n2)C2=NC(c3ccccc3)=CCN12
C-S(=O)(=O)-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[#7;a:4]:[c:5].[C:6]-[C:7](-[C;D1;H3:8])-[NH2;D1;+0:9]>>[C:6]-[C:7](-[C;D1;H3:8])-[NH;D2;+0:9]-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[#7;a:4]:[c:5]
null
[]
null
null
null
null
1-(2-methanesulfonyl-pyrimidin-4-yl)-8-phenyl-1,2,3,6-tetrahydro-pyrimido[1,2-a]pyrimidin-4-one (1.1 g, 2.9 mmol) and [4-(2-amino-propyl)-phenyl]-methanol (0.96 g, 5.8 mmol) in 1:1 dioxane: 1-methyl-2-pyrrolidinone (16 mL) was heated to 100° C. for 20 h. The mixture was partitioned between water (30 mL) and ethyl aceta...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cncnc1
c1cncnc1
c1ccccc1.c1cncnc1.C1=CN=C2[NH]CCCN2C1.c1ccccc1
HO-
CN1C(CCC1)=O
null
null
CC(N)Cc1ccc(CO)cc1.CS(=O)(=O)c1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1>CN1C(CCC1)=O>CC(Cc1ccc(CO)cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-520a25fcf6cc443b94c8b137ba59102e
CC(Cc1ccc(CO)cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1.[N-]=[N+]=NP(=O)(c1ccccc1)c1ccccc1>>CC(Cc1ccc(CN=[N+]=[N-])cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
OCC1=CC=C(C=C1)CC(C)NC1=NC=CC(=N1)N1C=2N(C(CC1)=O)CC=C(N2)C2=CC=CC=C2.N12CCCCCC2=NCCC1.C1(=CC=CC=C1)P(=O)(C1=CC=CC=C1)N=[N+]=[N-]>>N(=[N+]=[N-])CC1=CC=C(C=C1)CC(C)NC1=NC=CC(=N1)N1C=2N(C(CC1)=O)CC=C(N2)C2=CC=CC=C2
O[CH2:8][c:7]1[cH:6][cH:5][c:4]([CH2:3][CH:2]([CH3:1])[NH:14][c:15]2[n:16][cH:17][cH:18][c:19]([N:20]3[CH2:21][CH2:22][C:23](=[O:24])[N:25]4[CH2:26][CH:27]=[C:28]([c:29]5[cH:30][cH:31][cH:32][cH:33][cH:34]5)[N:35]=[C:36]34)[n:37]2)[cH:13][cH:12]1.O=P(c1ccccc1)(c1ccccc1)[N:9]=[N+:10]=[N-:11]>>[CH3:1][CH:2]([CH2:3][c:4]1...
CC(Cc1ccc(CO)cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1.[N-]=[N+]=NP(=O)(c1ccccc1)c1ccccc1
CC(Cc1ccc(CN=[N+]=[N-])cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
null
null
O1CCCC1
Heteroatom Alkylation and Arylation
OtherReaction
cfa52427fe008248ccb3b060cca934c64c46f29eb11684ddb953f16825bf2f0e
da5ad8c0affa2dc7232b479927687ff59fae3f37df63d467193897a964229798
O=C1CCN(c2ccnc(NCCc3ccccc3)n2)C2=NC(c3ccccc3)=CCN12
O-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].O=P(-[N;H0;D2;+0:5]=[#7;+:6]=[N;-;D1;H0:7])(-c1:c:c:c:c:c:1)-c1:c:c:c:c:c:1>>[N;-;D1;H0:7]=[#7;+:6]=[N;H0;D2;+0:5]-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
17
HOUR
The mixture of 1-{2-[2-(4-hydroxymethyl-phenyl)-1-methyl-ethylamino]-pyrimidin-4-yl}-8-phenyl-1,2,3,6-tetrahydro -pyrimido[1,2-a]pyrimidin-4-one (0.11 g, 0.24 mmol) and 1,8-diaza-bicyclo[5.4.0]undec-7-ene (47 μL, 0.312 mmol) in tetrahydrofuran (5 mL) was brought to 0° C. followed by the addition of diphenylphosphoryl a...
10.6084/m9.figshare.5104873.v1
null
Azide.Primary alcohol
Azide
c1ccccc1.c1ccccc1
null
c1ccccc1.c1cncnc1.C1=CN=C2[NH]CCCN2C1.c1ccccc1
HO-
O1CCCC1
null
17
CC(Cc1ccc(CO)cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1.[N-]=[N+]=NP(=O)(c1ccccc1)c1ccccc1>O1CCCC1>CC(Cc1ccc(CN=[N+]=[N-])cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8ac111c1e0264127af1000863e1571da
CC(Cc1ccc(CN=[N+]=[N-])cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1>>CC(Cc1ccc(CN)cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
N(=[N+]=[N-])CC1=CC=C(C=C1)CC(C)NC1=NC=CC(=N1)N1C=2N(C(CC1)=O)CC=C(N2)C2=CC=CC=C2.C1=CCC=CC1>>NCC1=CC=C(C=C1)CC(C)NC1=NC=CC(=N1)N1C=2N(C(CC1)=O)CC=C(N2)C2=CC=CC=C2
[N-]=[N+]=[N:9][CH2:8][c:7]1[cH:6][cH:5][c:4]([CH2:3][CH:2]([CH3:1])[NH:12][c:13]2[n:14][cH:15][cH:16][c:17]([N:18]3[CH2:19][CH2:20][C:21](=[O:22])[N:23]4[CH2:24][CH:25]=[C:26]([c:27]5[cH:28][cH:29][cH:30][cH:31][cH:32]5)[N:33]=[C:34]34)[n:35]2)[cH:11][cH:10]1>>[CH3:1][CH:2]([CH2:3][c:4]1[cH:5][cH:6][c:7]([CH2:8][NH2:9...
CC(Cc1ccc(CN=[N+]=[N-])cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
CC(Cc1ccc(CN)cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
null
[Pd]
C(C)OC(C)=O
Reduction
Azide to amine reduction (Staudinger)
4c9e4990dae2bb965dec06bd45e318560989ee3681b61e443f7aa363b7cfa222
cd009d687d606bf351eac9390a176d16be38f2c8216a599b398641009c215027
O=C1CCN(c2ccnc(NCCc3ccccc3)n2)C2=NC(c3ccccc3)=CCN12
[N-]=[N+]=[N;H0;D2;+0:1]-[C:2]-[c:3]>>[NH2;D1;+0:1]-[C:2]-[c:3]
null
[]
null
null
null
null
The mixture of 1-{2-[2-(4-azidomethyl-phenyl)-1-methyl-ethylamino]-pyrimidin-4-yl}-8-phenyl-1,2,3,6-tetrahydro-pyrimido[1,2-a]pyrimidin-4-one, 1,4-cyclohexadiene (80 μL, 0.80 mmol) and palladium on carbon (100 mg) in ethylacetate (10 mL) was heated to reflux for 3 h and brought to room temperature. The mixture was filt...
10.6084/m9.figshare.5104873.v1
null
Azide
Primary amine
null
null
c1ccccc1.c1cncnc1.C1=CN=C2[NH]CCCN2C1.c1ccccc1
Other
[Pd].C(C)OC(C)=O
null
null
CC(Cc1ccc(CN=[N+]=[N-])cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1>[Pd].C(C)OC(C)=O>CC(Cc1ccc(CN)cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6de1fbcc324e4549a960abe50ca5c371
CC(Cc1ccc(CO)cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1>>CC(Cc1ccc(C=O)cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
OCC1=CC=C(C=C1)CC(C)NC1=NC=CC(=N1)N1C=2N(C(CC1)=O)CC=C(N2)C2=CC=CC=C2>>O=C1CCN(C=2N1CC=C(N2)C2=CC=CC=C2)C2=NC(=NC=C2)NC(CC2=CC=C(C=O)C=C2)C
[CH3:1][CH:2]([CH2:3][c:4]1[cH:5][cH:6][c:7]([CH2:8][OH:9])[cH:10][cH:11]1)[NH:12][c:13]1[n:14][cH:15][cH:16][c:17]([N:18]2[CH2:19][CH2:20][C:21](=[O:22])[N:23]3[CH2:24][CH:25]=[C:26]([c:27]4[cH:28][cH:29][cH:30][cH:31][cH:32]4)[N:33]=[C:34]23)[n:35]1>>[CH3:1][CH:2]([CH2:3][c:4]1[cH:5][cH:6][c:7]([CH:8]=[O:9])[cH:10][c...
CC(Cc1ccc(CO)cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
CC(Cc1ccc(C=O)cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
null
[O-2].[O-2].[Mn+4]
ClCCl
Oxidation
Oxidation or Dehydrogenation of Alcohols to Aldehydes and Ketones
41bfa9deea81b465c88ad21fdfb64a2e1ba29490558cf430df132cb98b4a538b
0a03c6724c1862e8f86d4a463afda55b8e067dc6cb42597b472eb7cabc03eda3
O=C1CCN(c2ccnc(NCCc3ccccc3)n2)C2=NC(c3ccccc3)=CCN12
[OH;D1;+0:1]-[CH2;D2;+0:2]-[c:3](:[c:4]):[c:5]>>[O;H0;D1;+0:1]=[CH;D2;+0:2]-[c:3](:[c:4]):[c:5]
null
[]
null
null
3
HOUR
The mixture of 1-{2-[2-(4-hydroxymethyl-phenyl)-1-methyl-ethylamino]-pyrimidin-4-yl}-8-phenyl-1,2,3,6-tetrahydro -pyrimido[1,2-a]pyrimidin-4-one (0.38 g, 0.81 mmol) and manganese dioxide (3.5 g, 40.5 mmol) in dichloromethane was stirred at room temperature for 3 h. The mixture was filtered off and concentrated to affor...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Aldehyde
null
null
c1ccccc1.c1cncnc1.C1=CN=C2[NH]CCCN2C1.c1ccccc1
null
[O-2].[O-2].[Mn+4].ClCCl
null
3
CC(Cc1ccc(CO)cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1>[O-2].[O-2].[Mn+4].ClCCl>CC(Cc1ccc(C=O)cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-fe623d6467d644408b59e4f27cf4bf16
CC(Cc1ccc(C=O)cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1.CC[N+](=O)[O-]>>CC(=Cc1ccc(CC(C)Nc2nccc(N3CCC(=O)N4CC=C(c5ccccc5)N=C43)n2)cc1)[N+](=O)[O-]
O=C1CCN(C=2N1CC=C(N2)C2=CC=CC=C2)C2=NC(=NC=C2)NC(CC2=CC=C(C=O)C=C2)C.C(C)(=O)[O-].[NH4+].[N+](=O)([O-])CC>>CC(CC1=CC=C(C=C1)C=C(C)[N+](=O)[O-])NC1=NC=CC(=N1)N1C=2N(C(CC1)=O)CC=C(N2)C2=CC=CC=C2
O=[CH:3][c:4]1[cH:5][cH:6][c:7]([CH2:8][CH:9]([CH3:10])[NH:11][c:12]2[n:13][cH:14][cH:15][c:16]([N:17]3[CH2:18][CH2:19][C:20](=[O:21])[N:22]4[CH2:23][CH:24]=[C:25]([c:26]5[cH:27][cH:28][cH:29][cH:30][cH:31]5)[N:32]=[C:33]34)[n:34]2)[cH:35][cH:36]1.[CH3:1][CH2:2][N+:37](=[O:38])[O-:39]>>[CH3:1][C:2](=[CH:3][c:4]1[cH:5][...
CC(Cc1ccc(C=O)cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1.CC[N+](=O)[O-]
CC(=Cc1ccc(CC(C)Nc2nccc(N3CCC(=O)N4CC=C(c5ccccc5)N=C43)n2)cc1)[N+](=O)[O-]
null
null
null
C-C Coupling
OtherReaction
7ede86d40d3d69f429dde089476c8b7ffa9b74bf3050590255e6323d013c2daf
f736727903c0ad5511d468246b8e380897fd19905174c118ffa4ed4d3651f6ea
O=C1CCN(c2ccnc(NCCc3ccccc3)n2)C2=NC(c3ccccc3)=CCN12
O=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4].[C;D1;H3:5]-[CH2;D2;+0:6]-[#7;+:7](-[O;-;D1;H0:8])=[O;D1;H0:9]>>[C;D1;H3:5]-[C;H0;D3;+0:6](=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4])-[#7;+:7](-[O;-;D1;H0:8])=[O;D1;H0:9]
null
[]
null
null
null
null
The mixture of 4-{2-[4-(4-oxo-8-phenyl-3,4-dihydro-2H,6H-pyrimido[1,2-a]pyrimidin-1-yl) -pyrimidin-2-ylamino]-propyl}-benzaldehyde (35 mg, 0.08 mmol), ammonium acetate (10 mg, 0.16 mmol) in nitroethane (5 mL) was heated to reflux for 4 h. The mixture was brought to room temperature and concentrated. The residue was dis...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Nitro group
Enamine
null
null
c1ccccc1.c1cncnc1.C1=CN=C2[NH]CCCN2C1.c1ccccc1
HO-
null
null
null
CC(Cc1ccc(C=O)cc1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1.CC[N+](=O)[O-]>>CC(=Cc1ccc(CC(C)Nc2nccc(N3CCC(=O)N4CC=C(c5ccccc5)N=C43)n2)cc1)[N+](=O)[O-]
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-18ca248961c84170805d4e3148ba8a0c
CC(=Cc1ccc(CC(C)Nc2nccc(N3CCC(=O)N4CC=C(c5ccccc5)N=C43)n2)cc1)[N+](=O)[O-]>>CC(N)Cc1ccc(CC(C)Nc2nccc(N3CCC(=O)N4CC=C(c5ccccc5)N=C43)n2)cc1
CC(CC1=CC=C(C=C1)C=C(C)[N+](=O)[O-])NC1=NC=CC(=N1)N1C=2N(C(CC1)=O)CC=C(N2)C2=CC=CC=C2>>NC(CC1=CC=C(C=C1)CC(C)NC1=NC=CC(=N1)N1C=2N(C(CC1)=O)CC=C(N2)C2=CC=CC=C2)C
O=[N+:3]([O-])[C:2]([CH3:1])=[CH:4][c:5]1[cH:6][cH:7][c:8]([CH2:9][CH:10]([CH3:11])[NH:12][c:13]2[n:14][cH:15][cH:16][c:17]([N:18]3[CH2:19][CH2:20][C:21](=[O:22])[N:23]4[CH2:24][CH:25]=[C:26]([c:27]5[cH:28][cH:29][cH:30][cH:31][cH:32]5)[N:33]=[C:34]34)[n:35]2)[cH:36][cH:37]1>>[CH3:1][CH:2]([NH2:3])[CH2:4][c:5]1[cH:6][c...
CC(=Cc1ccc(CC(C)Nc2nccc(N3CCC(=O)N4CC=C(c5ccccc5)N=C43)n2)cc1)[N+](=O)[O-]
CC(N)Cc1ccc(CC(C)Nc2nccc(N3CCC(=O)N4CC=C(c5ccccc5)N=C43)n2)cc1
null
[Pd]
CO
Reduction
OtherReaction
4337e4e8b75c4193a30be38c3139251eb50201a1e90dac1ecfc293dd3e226a46
1ad3bfd18d4cba7c52a6c2c4705cfa4e2dc99589d9555154a809489f21a7a436
O=C1CCN(c2ccnc(NCCc3ccccc3)n2)C2=NC(c3ccccc3)=CCN12
O=[N+;H0;D3:1](-[O-])-[C;H0;D3;+0:2](-[C;D1;H3:3])=[CH;D2;+0:4]-[c:5](:[c:6]):[c:7]>>[C;D1;H3:3]-[CH;D3;+0:2](-[NH2;D1;+0:1])-[CH2;D2;+0:4]-[c:5](:[c:6]):[c:7]
null
[]
null
null
null
null
Through a mixture of 1-(2-{1-methyl-2-[4-(2-nitro-propenyl)-phenyl]-ethylamino}-pyrimidin-4-yl)-8-phenyl-1,2,3,6-tetrahydro-pyrimido[1,2-a]pyrimidin-4-one (10 mg, 0.02 mmol) and palladium on carbon (cat) in methanol was bubbled hydrogen through a balloon for 17 h. The mixure was filtered through celite, concentrated an...
10.6084/m9.figshare.5104873.v1
null
Enamine
Primary amine
null
null
c1ccccc1.c1cncnc1.C1=CN=C2[NH]CCCN2C1.c1ccccc1
Other
[Pd].CO
null
null
CC(=Cc1ccc(CC(C)Nc2nccc(N3CCC(=O)N4CC=C(c5ccccc5)N=C43)n2)cc1)[N+](=O)[O-]>[Pd].CO>CC(N)Cc1ccc(CC(C)Nc2nccc(N3CCC(=O)N4CC=C(c5ccccc5)N=C43)n2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c8818ae657bd4d0dacbe9faef226530c
CC(C)(O)c1cccc(Br)c1.N#CCCl.O=S(=O)(O)O>>CC(C)(NC(=O)CCl)c1cccc(Br)c1
BrC=1C=C(C=CC1)C(C)(C)O.ClCC#N.S(O)(O)(=O)=O>>BrC=1C=C(C=CC1)C(C)(C)NC(CCl)=O
O[C:2]([CH3:1])([CH3:3])[c:9]1[cH:10][cH:11][cH:12][c:13]([Br:14])[cH:15]1.[N:4]#[C:5][CH2:7][Cl:8].O=S(=O)(O)[OH:6]>>[CH3:1][C:2]([CH3:3])([NH:4][C:5](=[O:6])[CH2:7][Cl:8])[c:9]1[cH:10][cH:11][cH:12][c:13]([Br:14])[cH:15]1
CC(C)(O)c1cccc(Br)c1.N#CCCl.O=S(=O)(O)O
CC(C)(NC(=O)CCl)c1cccc(Br)c1
null
null
C(C)(=O)O
Heteroatom Alkylation and Arylation
OtherReaction
1d5b8ab7abc796c8fe1a4bbe88d643f3667784ffa1e5d5bdf2ecec75239c4174
351ef33c26e45ccdbae92f97c6925d748e3ebc471a863d8f431e8ded2d7e850d
c1ccccc1
O-S(=O)(=O)-[OH;D1;+0:1].O-[C;H0;D4;+0:2](-[C;D1;H3:3])(-[C;D1;H3:4])-[c:5](:[c:6]):[c:7].[Cl;D1;H0:8]-[C:9]-[C;H0;D2;+0:10]#[N;H0;D1;+0:11]>>[C;D1;H3:3]-[C;H0;D4;+0:2](-[C;D1;H3:4])(-[NH;D2;+0:11]-[C;H0;D3;+0:10](=[O;H0;D1;+0:1])-[C:9]-[Cl;D1;H0:8])-[c:5](:[c:6]):[c:7]
null
[]
0
CELSIUS
17
HOUR
To a mixture of the 2-(3-bromo-phenyl)-propan-2-ol and (0.76 g, 3.6 mmol) and chloro-acetonitrile (7 mL) was added acetic acid (0.6 mL) and the resulting mixture was cooled to 0° C. Concentrated sulfuric acid (0.6 mL) was added dropwise and the mixture was brought to room temperature and stirred for 17 h. Mixture was p...
10.6084/m9.figshare.5104873.v1
null
Nitrile.Tertiary alcohol
Secondary amide
null
null
c1ccccc1
HO-
C(C)(=O)O
0
17
CC(C)(O)c1cccc(Br)c1.N#CCCl.O=S(=O)(O)O>C(C)(=O)O>CC(C)(NC(=O)CCl)c1cccc(Br)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c93c2c43beef47f48b7d8aba95b9eaec
CC(C)(NC(=O)CCl)c1cccc(Br)c1>>CC(C)(N)c1cccc(Br)c1
O.BrC=1C=C(C=CC1)C(C)(C)NC(CCl)=O.NC(=S)N.C(C)(=O)O>>BrC=1C=C(C=CC1)C(C)(C)N
O=C(CCl)[NH:4][C:2]([CH3:1])([CH3:3])[c:5]1[cH:6][cH:7][cH:8][c:9]([Br:10])[cH:11]1>>[CH3:1][C:2]([CH3:3])([NH2:4])[c:5]1[cH:6][cH:7][cH:8][c:9]([Br:10])[cH:11]1
CC(C)(NC(=O)CCl)c1cccc(Br)c1
CC(C)(N)c1cccc(Br)c1
null
null
C(C)O
Reduction
Hydrogenolysis of amides/imides/carbamates
807b1f1939ea7d761c5d620a58a82fc0384736a2623a6465702aec6b6eafca82
2e2d3841e5ab0432159afeb516096047b79f5ff710ff12d384f8f6e373d52484
c1ccccc1
Cl-C-C(=O)-[NH;D2;+0:1]-[C:2](-[C;D1;H3:3])(-[C;D1;H3:4])-[c:5]>>[C;D1;H3:3]-[C:2](-[C;D1;H3:4])(-[NH2;D1;+0:1])-[c:5]
null
[]
null
null
null
null
The mixture of N-[1-(3-bromo-phenyl)-1-methyl-ethyl]-2-chloro-acetamide (1.0 g, 3.5 mmol), thiourea (0.32 g, 4.2 mmol), acetic acid (1.5 mL) in ethanol (7 mL) was heated to reflux for 10 h and brought to room temperature. Water was added to the mixture until a precipitate was formed which was filtered. The filtrate was...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amide
Primary amine
null
null
c1ccccc1
HCl
C(C)O
null
null
CC(C)(NC(=O)CCl)c1cccc(Br)c1>C(C)O>CC(C)(N)c1cccc(Br)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-82f70b5da0c44140bd1eb2eb0d078c06
C=CC(=O)OCC.CC(C)(N)c1cccc(Br)c1.CN(C1CCCCC1)C1CCCCC1>>COC(=O)C(C)=Cc1cccc(C(C)(C)N)c1
C(C=C)(=O)OCC.C(C)(C)(C)P(C(C)(C)C)C(C)(C)C.BrC=1C=C(C=CC1)C(C)(C)N.CN(C1CCCCC1)C1CCCCC1>>COC(C(=CC1=CC(=CC=C1)C(C)(C)N)C)=O
C[CH2:1][O:2][C:3](=[O:4])[CH:5]=[CH2:6].Br[c:8]1[cH:9][cH:10][cH:11][c:12]([C:13]([CH3:14])([CH3:15])[NH2:16])[cH:17]1.CN(C1CCCCC1)C1CCCC[CH2:7]1>>[CH3:1][O:2][C:3](=[O:4])[C:5]([CH3:6])=[CH:7][c:8]1[cH:9][cH:10][cH:11][c:12]([C:13]([CH3:14])([CH3:15])[NH2:16])[cH:17]1
C=CC(=O)OCC.CC(C)(N)c1cccc(Br)c1.CN(C1CCCCC1)C1CCCCC1
COC(=O)C(C)=Cc1cccc(C(C)(C)N)c1
null
C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd]
O1CCOCC1.O
C-C Coupling
OtherReaction
206806302ed78190ad75d1f786fc14274f4bbd23851875e21565ae44e45d1e3c
8e0661f9e28121ac6c2a1c7506a439ed7a76b37b3cf9ee523f78f73fb18e012e
c1ccccc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].C-N(-C1-C-C-C-C-C-1)-C1-C-C-C-C-[CH2;D2;+0:6]-1.C-[CH2;D2;+0:7]-[#8:8]-[C:9](=[O;D1;H0:10])-[CH;D2;+0:11]=[CH2;D1;+0:12]>>[CH3;D1;+0:7]-[#8:8]-[C:9](=[O;D1;H0:10])-[C;H0;D3;+0:11](-[CH3;D1;+0:12])=[CH;D2;+0:6]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
null
[]
80
CELSIUS
null
null
The mixture of 1-(3-bromo-phenyl)-1-methyl-ethylamine (0.74 g, 3.5 mmol), tris(dibenzylideneacetone)dipalladium (0.19 g, 0.21 mmol), and N-methyldicyclohexylamine (10 mmol) was purged with nitrogen followed by the addition of 1,4-dioxane (7 mL) and tri-tert-butylphospine (85 mg, 0.42 mmol). The mixture was again purged...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Tertiary amine.Vinyl
Ester
c1ccccc1.C1CCCCC1.C1CCCCC1
c1ccccc1
c1ccccc1
HBr
C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd].O1CCOCC1.O
80
null
C=CC(=O)OCC.CC(C)(N)c1cccc(Br)c1.CN(C1CCCCC1)C1CCCCC1>C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd].O1CCOCC1.O>COC(=O)C(C)=Cc1cccc(C(C)(C)N)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-69ee3bd99eda4cc58d6d1e27af82a7af
COC(=O)C(C)=Cc1cccc(C(C)(C)N)c1>>COC(=O)C(C)Cc1cccc(C(C)(C)N)c1
COC(C(=CC1=CC(=CC=C1)C(C)(C)N)C)=O.[Mg]>>COC(C(CC1=CC(=CC=C1)C(C)(C)N)C)=O
[CH3:1][O:2][C:3](=[O:4])[C:5]([CH3:6])=[CH:7][c:8]1[cH:9][cH:10][cH:11][c:12]([C:13]([CH3:14])([CH3:15])[NH2:16])[cH:17]1>>[CH3:1][O:2][C:3](=[O:4])[CH:5]([CH3:6])[CH2:7][c:8]1[cH:9][cH:10][cH:11][c:12]([C:13]([CH3:14])([CH3:15])[NH2:16])[cH:17]1
COC(=O)C(C)=Cc1cccc(C(C)(C)N)c1
COC(=O)C(C)Cc1cccc(C(C)(C)N)c1
null
null
CO
Reduction
Hydrogenation (double to single)
c04c38f95d7b746e5bdb99c368a7a33956c97b95b54c7ad89be2a85526386ec9
9a50abf8d2e4cd9195d7a0cadbe97483a261a81cf70b653cfddd5ecf76d383a6
c1ccccc1
[C;D1;H3:1]-[#8:2]-[C:3](=[O;D1;H0:4])-[C;H0;D3;+0:5](-[C;D1;H3:6])=[CH;D2;+0:7]-[c:8](:[c:9]):[c:10]>>[C;D1;H3:1]-[#8:2]-[C:3](=[O;D1;H0:4])-[CH;D3;+0:5](-[C;D1;H3:6])-[CH2;D2;+0:7]-[c:8](:[c:9]):[c:10]
null
[]
null
null
null
null
The mixture of 3-[3-(1-amino-1-methyl-ethyl)-phenyl]-2-methylacrylic acid methyl ester (2.0 g, 8.6 mmol), magnesium (0.63 g, 25.8 mmol) in methanol was heated to reflux for 3 h until the starting material was consumed. The mixture was brought to room temperature, filtered and the filtrate was concentrated. The residue ...
10.6084/m9.figshare.5104873.v1
null
Ester
Ester
null
null
c1ccccc1
null
CO
null
null
COC(=O)C(C)=Cc1cccc(C(C)(C)N)c1>CO>COC(=O)C(C)Cc1cccc(C(C)(C)N)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9a439986ea774601a847d5a4ee6fdaee
CC(Cc1cccc(C(C)(C)NC(=O)OC(C)(C)C)c1)NC(=O)OCc1ccccc1>>CC(N)Cc1cccc(C(C)(C)NC(=O)OC(C)(C)C)c1
C(C)(C)(C)OC(NC(C)(C)C1=CC(=CC=C1)CC(C)NC(=O)OCC1=CC=CC=C1)=O.C1=CCC=CC1>>C(C)(C)(C)OC(NC(C)(C)C1=CC(=CC=C1)CC(C)N)=O
O=C(OCc1ccccc1)[NH:3][CH:2]([CH3:1])[CH2:4][c:5]1[cH:6][cH:7][cH:8][c:9]([C:10]([CH3:11])([CH3:12])[NH:13][C:14](=[O:15])[O:16][C:17]([CH3:18])([CH3:19])[CH3:20])[cH:21]1>>[CH3:1][CH:2]([NH2:3])[CH2:4][c:5]1[cH:6][cH:7][cH:8][c:9]([C:10]([CH3:11])([CH3:12])[NH:13][C:14](=[O:15])[O:16][C:17]([CH3:18])([CH3:19])[CH3:20])...
CC(Cc1cccc(C(C)(C)NC(=O)OC(C)(C)C)c1)NC(=O)OCc1ccccc1
CC(N)Cc1cccc(C(C)(C)NC(=O)OC(C)(C)C)c1
null
[Pd]
CO
Reduction
Hydrogenolysis of amides/imides/carbamates
087b6600ba91d3df931fe6979f2445c192cbfd59e04fd2d8a10f7c7573ac669f
4e549866ec1acadec4c84aaf8495992a28ec78d8ea5ef1b9f44dd843b0dcb7d4
c1ccccc1
O=C(-O-C-c1:c:c:c:c:c:1)-[NH;D2;+0:1]-[C:2](-[C:3])-[C;D1;H3:4]>>[C:3]-[C:2](-[C;D1;H3:4])-[NH2;D1;+0:1]
null
[]
null
null
null
null
To a mixture of {1-[3-(2-benzyloxycarbonylamino-propyl)-phenyl]-1-methyl-ethyl}-carbamic acid tert-butyl ester (0.28 g, 0.65 mmol), 1,4-cyclohexadiene (0.31 mL, 3.25 mmol) and Pd/C (cat.) in methanol was heated to reflux for 17 h. The mixture was filtered through celite and concentrated to afford light yellow oil. M+1=...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether
Primary amine
c1ccccc1
null
c1ccccc1
HO-
[Pd].CO
null
null
CC(Cc1cccc(C(C)(C)NC(=O)OC(C)(C)C)c1)NC(=O)OCc1ccccc1>[Pd].CO>CC(N)Cc1cccc(C(C)(C)NC(=O)OC(C)(C)C)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ff635817f03644f0ba08ecbb08762b29
CC(N)Cc1cccc(C(C)(C)NC(=O)OC(C)(C)C)c1.CS(=O)(=O)c1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1>>CC(Cc1cccc(C(C)(C)NC(=O)OC(C)(C)C)c1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
C(C)(C)(C)OC(NC(C)(C)C1=CC(=CC=C1)CC(C)N)=O.CS(=O)(=O)C1=NC=CC(=N1)N1C=2N(C(CC1)=O)CC=C(N2)C2=CC=CC=C2.O>>C(C)(C)(C)OC(NC(C)(C1=CC(=CC=C1)CC(C)NC1=NC=CC(=N1)N1C=2N(C(CC1)=O)CC=C(N2)C2=CC=CC=C2)C)=O
[CH3:1][CH:2]([CH2:3][c:4]1[cH:5][cH:6][cH:7][c:8]([C:9]([CH3:10])([CH3:11])[NH:12][C:13](=[O:14])[O:15][C:16]([CH3:17])([CH3:18])[CH3:19])[cH:20]1)[NH2:21].CS(=O)(=O)[c:22]1[n:23][cH:24][cH:25][c:26]([N:27]2[CH2:28][CH2:29][C:30](=[O:31])[N:32]3[CH2:33][CH:34]=[C:35]([c:36]4[cH:37][cH:38][cH:39][cH:40][cH:41]4)[N:42]=...
CC(N)Cc1cccc(C(C)(C)NC(=O)OC(C)(C)C)c1.CS(=O)(=O)c1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
CC(Cc1cccc(C(C)(C)NC(=O)OC(C)(C)C)c1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
null
null
CN1CCCC1=O
Heteroatom Alkylation and Arylation
OtherReaction
289adcacbe89f1503fb3c9d1b660927aaeb421d7b5520077738f22dce3010144
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=C1CCN(c2ccnc(NCCc3ccccc3)n2)C2=NC(c3ccccc3)=CCN12
C-S(=O)(=O)-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[#7;a:4]:[c:5].[C:6]-[C:7](-[C;D1;H3:8])-[NH2;D1;+0:9]>>[C:6]-[C:7](-[C;D1;H3:8])-[NH;D2;+0:9]-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[#7;a:4]:[c:5]
null
[]
100
CELSIUS
null
null
To a mixture of {1-[3-(2-amino-propyl)-phenyl]-1-methyl -ethyl}-carbamic acid tert-butyl ester (0.19 g, 0.65 mmol) and 1-(2-methanesulfonyl-pyrimidin-4-yl) -8-phenyl-1,2,3,6-tetrahydro-pyrimido[1,2-a]pyrimidin-4-one (0.26 g, 0.72 mmol) in NMP (2 mL) was heated to 100° C. for 17 h. The mixture was poured into water (15 ...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cncnc1
c1cncnc1
c1ccccc1.c1cncnc1.C1=CN=C2[NH]CCCN2C1.c1ccccc1
HO-
CN1CCCC1=O
100
null
CC(N)Cc1cccc(C(C)(C)NC(=O)OC(C)(C)C)c1.CS(=O)(=O)c1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1>CN1CCCC1=O>CC(Cc1cccc(C(C)(C)NC(=O)OC(C)(C)C)c1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-87085bbfff944db9bf5d4bd3f1482fe7
CC(Cc1cccc(C(C)(C)NC(=O)OC(C)(C)C)c1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1>>CC(Cc1cccc(C(C)(C)N)c1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
C(C)(C)(C)OC(NC(C)(C1=CC(=CC=C1)CC(C)NC1=NC=CC(=N1)N1C=2N(C(CC1)=O)CC=C(N2)C2=CC=CC=C2)C)=O.FC(C(=O)O)(F)F>>NC(C)(C)C=1C=C(C=CC1)CC(C)NC1=NC=CC(=N1)N1C=2N(C(CC1)=O)CC=C(N2)C2=CC=CC=C2
CC(C)(C)OC(=O)[NH:12][C:9]([c:8]1[cH:7][cH:6][cH:5][c:4]([CH2:3][CH:2]([CH3:1])[NH:14][c:15]2[n:16][cH:17][cH:18][c:19]([N:20]3[CH2:21][CH2:22][C:23](=[O:24])[N:25]4[CH2:26][CH:27]=[C:28]([c:29]5[cH:30][cH:31][cH:32][cH:33][cH:34]5)[N:35]=[C:36]34)[n:37]2)[cH:13]1)([CH3:10])[CH3:11]>>[CH3:1][CH:2]([CH2:3][c:4]1[cH:5][c...
CC(Cc1cccc(C(C)(C)NC(=O)OC(C)(C)C)c1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
CC(Cc1cccc(C(C)(C)N)c1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
null
null
ClCCl
Reduction
Hydrogenolysis of amides/imides/carbamates
3c33dd2a2d355ee5ba0287367e209aa147a39aa00607f0c95fb2bf1ade45d014
c5b5dffe7dd8beebdc1baa8b5b05300a9f7079e65dcfd42ade6f8a77ff09537d
O=C1CCN(c2ccnc(NCCc3ccccc3)n2)C2=NC(c3ccccc3)=CCN12
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[C:2](-[C;D1;H3:3])(-[C;D1;H3:4])-[c:5]>>[C;D1;H3:3]-[C:2](-[C;D1;H3:4])(-[NH2;D1;+0:1])-[c:5]
null
[]
null
null
30
MINUTE
To a mixture of [1-methyl-1-(3-{2-[4-(4-oxo-8-phenyl-3,4-dihydro-2H, 6H-pyrimido[1,2-a]pyrimidin-1-yl)-pyrimidin-2-ylamino]-propyl}-phenyl)-ethyl]-carbamic acid tert-butyl ester (0.25 g, 0.42 mmol) and trifluoroacetic acid (1 mL) in dichloromethane (2 mL) was stirred at room temperature for 30 min. The mixture was wash...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Primary amine
null
null
c1ccccc1.c1cncnc1.C1=CN=C2[NH]CCCN2C1.c1ccccc1
HO-
ClCCl
null
0.5
CC(Cc1cccc(C(C)(C)NC(=O)OC(C)(C)C)c1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1>ClCCl>CC(Cc1cccc(C(C)(C)N)c1)Nc1nccc(N2CCC(=O)N3CC=C(c4ccccc4)N=C32)n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a93d0ed17ef24fb492871f8e95ea8aed
N=C(N)N.NCC(O)CN>>N=C1NCC(O)CN1
OC(CN)CN.Cl.NC(=N)N.CC(C)O>>Cl.N=C1NCC(CN1)O
N[C:3](N)=[NH:2].[NH2:4][CH2:5][CH:6]([OH:7])[CH2:8][NH2:9]>>[NH:2]=[C:3]1[NH:4][CH2:5][CH:6]([OH:7])[CH2:8][NH:9]1
N=C(N)N.NCC(O)CN
N=C1NCC(O)CN1
null
null
CC#N
Heteroatom Alkylation and Arylation
OtherReaction
884557aedb9ba33f3bd73c1a9f24022128ef861455c47665d1114455446729ad
9ad8d209678ee75009dc7068f43e3d0b5ea50e6f5b5deea7157a5815191d1c8b
N=C1NCCCN1
N-[C;H0;D3;+0:1](-N)=[N;D1;H1:2].[NH2;D1;+0:3]-[C:4]-[C:5]-[C:6]-[NH2;D1;+0:7]>>[N;D1;H1:2]=[C;H0;D3;+0:1]1-[NH;D2;+0:3]-[C:4]-[C:5]-[C:6]-[NH;D2;+0:7]-1
null
[]
140
CELSIUS
null
null
A mixture of 2-hydroxy -1,3-diaminopropane (9.80 g, 108 mmol) and guanidine hydrochloride (10.4 g, 108 mmol) in a 100 mL RBF was heated at 140° C. under nitrogen for 5 h. The reaction mixture, while under vigorous stirring, was let cooled to 100° C. whereby a mixture of iPrOH (5 mL) and CH3CN (5 mL) were added, resulti...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Primary amine.Primary amine.Primary amine
Secondary amine.Secondary amine
null
C1CNCNC1
C1CNCNC1
Other
CC#N
140
null
N=C(N)N.NCC(O)CN>CC#N>N=C1NCC(O)CN1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-53d91446c3054d59a42f9437d9e53686
CCOC(=O)CC(=O)c1ccccc1.N=C1NCC(O)CN1>>O=c1cc(-c2ccccc2)nc2n1CC(O)CN2
C(C)OC(CC(C1=CC=CC=C1)=O)=O.C(=O)([O-])[O-].[K+].[K+].Cl.N=C1NCC(CN1)O>>OC1CNC=2N(C(C=C(N2)C2=CC=CC=C2)=O)C1
CCO[C:2](=[O:1])[CH2:3][C:4](=O)[c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1.[NH:11]=[C:12]1[NH:13][CH2:14][CH:15]([OH:16])[CH2:17][NH:18]1>>[O:1]=[c:2]1[cH:3][c:4](-[c:5]2[cH:6][cH:7][cH:8][cH:9][cH:10]2)[n:11][c:12]2[n:13]1[CH2:14][CH:15]([OH:16])[CH2:17][NH:18]2
CCOC(=O)CC(=O)c1ccccc1.N=C1NCC(O)CN1
O=c1cc(-c2ccccc2)nc2n1CC(O)CN2
null
null
CCO
Aromatic Heterocycle Formation
OtherReaction
8f00f16f1c9d53f5f46d6d9a2025926fef0c98e92dd7de5b7a8939471e83a088
f590641b01cb525446469ed6ced5b738f453feb2f025056e9767d27c06e94b8b
O=c1cc(-c2ccccc2)nc2n1CCCN2
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[CH2;D2;+0:3]-[C;H0;D3;+0:4](=O)-[c;H0;D3;+0:5](:[c:6]:[c:7]):[c:8]:[c:9].[NH;D1;+0:10]=[C;H0;D3;+0:11]1-[#7:12]-[C:13]-[C:14]-[C:15]-[NH;D2;+0:16]-1>>[O;D1;H0:2]=[c;H0;D3;+0:1]1:[cH;D2;+0:3]:[c;H0;D3;+0:4](-[c;H0;D3;+0:5](:[c:6]:[c:7]):[c:8]:[c:9]):[n;H0;D2;+0:10]:[c;H0;D3;+0:11]2:[n...
null
[]
90
CELSIUS
17
HOUR
In a 250 mL RBF with a stirrer bar, a mixture of 3-oxo-3-phenyl-propionic acid ethyl ester (15 g, 78 mmol), K2CO3 (11.0 g, 80 mmol) and 2-imino-hexahydro-pyrimidin-5-ol hydrochloride (11.8 g, 78 mmol) in EtOH (150 mL) was heated at 90° C. under nitrogen overnight. After 17 h, the mixture was cooled to room temperature,...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ester.Secondary amine
null
C1CNCNC1
c1ccn2c(n1)NC[CH]C2
c1ccccc1.c1ccn2c(n1)NC[CH]C2
HO-
CCO
90
17
CCOC(=O)CC(=O)c1ccccc1.N=C1NCC(O)CN1>CCO>O=c1cc(-c2ccccc2)nc2n1CC(O)CN2
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-764a1ae4db054e5ea156281aaf351f1a
CC(C)(C)[Si](C)(C)OC1CN(c2ccnc(S(C)(=O)=O)n2)c2nc(-c3ccccc3)cc(=O)n2C1.C[C@H](N)c1ccccc1>>CC(Nc1nccc(N2CC(O[Si](C)(C)C(C)(C)C)Cn3c2nc(-c2ccccc2)cc3=O)n1)c1ccccc1
C(C)(C)(C)[Si](OC1CN(C=2N(C(C=C(N2)C2=CC=CC=C2)=O)C1)C1=NC(=NC=C1)S(=O)(=O)C)(C)C.C1(=CC=CC=C1)[C@H](C)N>>C(C)(C)(C)[Si](OC1CN(C=2N(C(C=C(N2)C2=CC=CC=C2)=O)C1)C1=NC(=NC=C1)NC(C)C1=CC=CC=C1)(C)C
CS(=O)(=O)[c:4]1[n:5][cH:6][cH:7][c:8]([N:9]2[CH2:10][CH:11]([O:12][Si:13]([CH3:14])([CH3:15])[C:16]([CH3:17])([CH3:18])[CH3:19])[CH2:20][n:21]3[c:22]2[n:23][c:24](-[c:25]2[cH:26][cH:27][cH:28][cH:29][cH:30]2)[cH:31][c:32]3=[O:33])[n:34]1.[CH3:1][C@H:2]([NH2:3])[c:35]1[cH:36][cH:37][cH:38][cH:39][cH:40]1>>[CH3:1][CH:2]...
CC(C)(C)[Si](C)(C)OC1CN(c2ccnc(S(C)(=O)=O)n2)c2nc(-c3ccccc3)cc(=O)n2C1.C[C@H](N)c1ccccc1
CC(Nc1nccc(N2CC(O[Si](C)(C)C(C)(C)C)Cn3c2nc(-c2ccccc2)cc3=O)n1)c1ccccc1
null
null
O1CCOCC1.CCOC(=O)C
Heteroatom Alkylation and Arylation
OtherReaction
289adcacbe89f1503fb3c9d1b660927aaeb421d7b5520077738f22dce3010144
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1cc(-c2ccccc2)nc2n1CCCN2c1ccnc(NCc2ccccc2)n1
C-S(=O)(=O)-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[#7;a:4]:[c:5].[C;D1;H3:6]-[C@H;D3;+0:7](-[NH2;D1;+0:8])-[c:9](:[c:10]):[c:11]>>[C;D1;H3:6]-[CH;D3;+0:7](-[NH;D2;+0:8]-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[#7;a:4]:[c:5])-[c:9](:[c:10]):[c:11]
null
[]
110
CELSIUS
null
null
A mixture of 7-(tert-butyl-dimethyl-silanyloxy)-9-(2-methanesulfonyl-pyrimidin-4-yl)-2-phenyl-6,7,8,9-tetrahydro-pyrimido[1,2-a]pyrimidin-4-one, prepared from last step (0.6 mmol) and (S)-1-phenylethylamine (1.0 mL, 7.8 mmol) in dioxane (6 mL) was heated at 110° C. for 17 h. The brown solution was cooled to room temper...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cncnc1
c1cncnc1
c1cncnc1.c1ccn2c(n1)NC[CH]C2.c1ccccc1.c1ccccc1
HO-
O1CCOCC1.CCOC(=O)C
110
null
CC(C)(C)[Si](C)(C)OC1CN(c2ccnc(S(C)(=O)=O)n2)c2nc(-c3ccccc3)cc(=O)n2C1.C[C@H](N)c1ccccc1>O1CCOCC1.CCOC(=O)C>CC(Nc1nccc(N2CC(O[Si](C)(C)C(C)(C)C)Cn3c2nc(-c2ccccc2)cc3=O)n1)c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-aa3c7d36b47c4cf790899e0a97557549
CC(Nc1nccc(N2CC(O[Si](C)(C)C(C)(C)C)Cn3c2nc(-c2ccccc2)cc3=O)n1)c1ccccc1>>CC(Nc1nccc(N2CC(O)Cn3c2nc(-c2ccccc2)cc3=O)n1)c1ccccc1
C(=O)(O)[O-].[Na+].C(C)(C)(C)[Si](OC1CN(C=2N(C(C=C(N2)C2=CC=CC=C2)=O)C1)C1=NC(=NC=C1)NC(C)C1=CC=CC=C1)(C)C.C(Cl)Cl.Cl>>OC1CN(C=2N(C(C=C(N2)C2=CC=CC=C2)=O)C1)C1=NC(=NC=C1)NC(C)C1=CC=CC=C1
CC(C)(C)[Si](C)(C)[O:12][CH:11]1[CH2:10][N:9]([c:8]2[cH:7][cH:6][n:5][c:4]([NH:3][CH:2]([CH3:1])[c:28]3[cH:29][cH:30][cH:31][cH:32][cH:33]3)[n:27]2)[c:15]2[n:14]([c:25](=[O:26])[cH:24][c:17](-[c:18]3[cH:19][cH:20][cH:21][cH:22][cH:23]3)[n:16]2)[CH2:13]1>>[CH3:1][CH:2]([NH:3][c:4]1[n:5][cH:6][cH:7][c:8]([N:9]2[CH2:10][C...
CC(Nc1nccc(N2CC(O[Si](C)(C)C(C)(C)C)Cn3c2nc(-c2ccccc2)cc3=O)n1)c1ccccc1
CC(Nc1nccc(N2CC(O)Cn3c2nc(-c2ccccc2)cc3=O)n1)c1ccccc1
null
null
CO
Deprotection
Alcohol deprotection from silyl ethers
050b4fb4e1e9936189860d27dded10ae70a294a642c52f800eb9d5aaef7955cc
88623e19d23cdfe8e1a4c167fd6cfc51d774a1c784b87a7bb2df8153ee93e67a
O=c1cc(-c2ccccc2)nc2n1CCCN2c1ccnc(NCc2ccccc2)n1
C-C(-C)(-C)-[Si](-C)(-C)-[O;H0;D2;+0:1]-[C:2](-[C:3]-[#7:4])-[C:5]-[#7;a:6]>>[#7:4]-[C:3]-[C:2](-[OH;D1;+0:1])-[C:5]-[#7;a:6]
null
[]
null
null
16
HOUR
A solution of 7-(tert-butyl-dimethyl-silanyloxy)-2-phenyl-9-[2-(1-phenyl-ethylamino)-pyrimidin-4-yl]-6,7,8,9-tetrahydro-pyrimido[1,2-a]pyrimidin-4-one (20 mg) in MeOH (3 mL)-DCM (1 mL) was treated with HCl (conc. 1.5 mL). After the mixture was stirred at room temperature for 16 h, it was neutralized with NaHCO3 (aq) an...
10.6084/m9.figshare.5104873.v1
null
TMS ether protective group
Secondary alcohol
null
null
c1cncnc1.c1ccn2c(n1)NC[CH]C2.c1ccccc1.c1ccccc1
Other
CO
null
16
CC(Nc1nccc(N2CC(O[Si](C)(C)C(C)(C)C)Cn3c2nc(-c2ccccc2)cc3=O)n1)c1ccccc1>CO>CC(Nc1nccc(N2CC(O)Cn3c2nc(-c2ccccc2)cc3=O)n1)c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ee5713a5f957405987c2c19d732f5004
CCOC(=O)CC(=CC#N)c1ccccc1.NCCN>>O=c1cc(-c2ccccc2)cc2n1CCN2
C(C)OC(CC(=CC#N)C1=CC=CC=C1)=O.C(CN)N>>C1(=CC=CC=C1)C=1C=C2N(C(C1)=O)CCN2
CCO[C:2](=[O:1])[CH2:3][C:4]([c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1)=[CH:11][C:12]#N.[NH2:13][CH2:14][CH2:15][NH2:16]>>[O:1]=[c:2]1[cH:3][c:4](-[c:5]2[cH:6][cH:7][cH:8][cH:9][cH:10]2)[cH:11][c:12]2[n:13]1[CH2:14][CH2:15][NH:16]2
CCOC(=O)CC(=CC#N)c1ccccc1.NCCN
O=c1cc(-c2ccccc2)cc2n1CCN2
null
null
null
Aromatic Heterocycle Formation
OtherReaction
f4c8ee0762a74d2b935553935519bf1eb02fcd52cc72bfe6895915070834faac
78e63bdc1504c9d55ec85b6a599f1cbdd667d3ae42ca4f82f3661c62d981c530
O=c1cc(-c2ccccc2)cc2n1CCN2
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[CH2;D2;+0:3]-[C;H0;D3;+0:4](=[CH;D2;+0:5]-[C;H0;D2;+0:6]#N)-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10]:[c:11].[NH2;D1;+0:12]-[C:13]-[C:14]-[NH2;D1;+0:15]>>[O;D1;H0:2]=[c;H0;D3;+0:1]1:[cH;D2;+0:3]:[c;H0;D3;+0:4](-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10]:[c:11]):[cH;D2;+0:5]:[c;H0;D3;+0:6]2:[n;H0;...
null
[]
160
CELSIUS
null
null
4-Cyano-3-phenyl-but-3-enoic acid ethyl ester (crude, 9.37 g, 0.043 mol), ethylenediamine (3 mL, 0.043 mol) were mixed in dichlorobenze (20 mL) and heated at 160° C. overnight. The resulting suspension was cooled to room temperature, filtered, and the filtrated cake was washed with EtOAc and finally dried to provide th...
10.6084/m9.figshare.5104873.v1
null
Ester.Nitrile.Primary amine.Primary amine
Secondary amine
null
c1ccn2c(c1)NCC2
c1ccccc1.c1ccn2c(c1)NCC2
HO-
null
160
null
CCOC(=O)CC(=CC#N)c1ccccc1.NCCN>>O=c1cc(-c2ccccc2)cc2n1CCN2
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4adc0ba0538a4090bb0ebdd5cc78d520
CSc1nccc(Cl)n1.O=c1cc(-c2ccccc2)cc2n1CCCN2>>CSc1nccc(N2CCCn3c2cc(-c2ccccc2)cc3=O)n1
ClC1=NC(=NC=C1)SC.C1(=CC=CC=C1)C=1C=C2N(CCCN2)C(C1)=O.CC(C)([O-])C.[Na+].C=1C=CC(=CC1)P(C=2C=CC=CC2)C3=CC=C4C=CC=CC4=C3C5=C6C=CC=CC6=CC=C5P(C=7C=CC=CC7)C=8C=CC=CC8>>CSC1=NC=CC(=N1)N1C=2N(CCC1)C(C=C(C2)C2=CC=CC=C2)=O
Cl[c:7]1[cH:6][cH:5][n:4][c:3]([S:2][CH3:1])[n:25]1.[NH:8]1[CH2:9][CH2:10][CH2:11][n:12]2[c:13]1[cH:14][c:15](-[c:16]1[cH:17][cH:18][cH:19][cH:20][cH:21]1)[cH:22][c:23]2=[O:24]>>[CH3:1][S:2][c:3]1[n:4][cH:5][cH:6][c:7]([N:8]2[CH2:9][CH2:10][CH2:11][n:12]3[c:13]2[cH:14][c:15](-[c:16]2[cH:17][cH:18][cH:19][cH:20][cH:21]2...
CSc1nccc(Cl)n1.O=c1cc(-c2ccccc2)cc2n1CCCN2
CSc1nccc(N2CCCn3c2cc(-c2ccccc2)cc3=O)n1
null
null
C1(=CC=CC=C1)C
Heteroatom Alkylation and Arylation
Ullmann-Goldberg Substitution amine
e4ffddb286271207ecd79dac97a88aa5f42eaa4284924638aeeb1b9d705dd954
b6b8e2cdb45054a35f5e8157d624f852c0601a09401556706e166b19536eb7a7
O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccncn1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](-[#16:4]):[#7;a:5]:[c:6]:[c:7]:1.[c:8]:[c:9]1:[#7;a:10](:[c:11])-[C:12]-[C:13]-[C:14]-[NH;D2;+0:15]-1>>[#16:4]-[c:3]1:[#7;a:2]:[c;H0;D3;+0:1](-[N;H0;D3;+0:15]2-[C:14]-[C:13]-[C:12]-[#7;a:10](:[c:11]):[c:9]-2:[c:8]):[c:7]:[c:6]:[#7;a:5]:1
null
[]
70
CELSIUS
null
null
To a mixture of 8-phenyl-1,2,3,4-tetrahydro-pyrido[1,2-a]pyrimidin-6-one (1.86 g, 8.23 mmol), sodium tert-butoxide (1.6 g, 16 mmol), BINAP (0.15 g, 0.207 mmol), and Pd (OAc)2 (55 mg, 0.2 mmol) was added toluene (20 mL) and 4-chloro -2-methylthiopyrimidine (1.5 mL, 12 mmol). After purged with N2 for 10 min, the overall ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Secondary amine
Tertiary amine
c1cncnc1.c1ccn2c(c1)NCCC2
c1cncnc1.c1ccn2c(c1)NCCC2
c1cncnc1.c1ccn2c(c1)NCCC2.c1ccccc1
HCl
C1(=CC=CC=C1)C
70
null
CSc1nccc(Cl)n1.O=c1cc(-c2ccccc2)cc2n1CCCN2>C1(=CC=CC=C1)C>CSc1nccc(N2CCCn3c2cc(-c2ccccc2)cc3=O)n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-18463e1b15a84f3184de7f73294a6b77
CSc1nccc(N2CCCn3c2cc(-c2ccccc2)cc3=O)n1.O=c1cc(-c2ccccc2)cc2n1CCN2>>CSc1nccc(N2CCn3c2cc(-c2ccccc2)cc3=O)n1
CSC1=NC=CC(=N1)N1C=2N(CCC1)C(C=C(C2)C2=CC=CC=C2)=O.CC(C)([O-])C.[Na+].C=1C=CC(=CC1)P(C=2C=CC=CC2)C3=CC=C4C=CC=CC4=C3C5=C6C=CC=CC6=CC=C5P(C=7C=CC=CC7)C=8C=CC=CC8.ClC1=NC(=NC=C1)SC.C1(=CC=CC=C1)C=1C=C2N(C(C1)=O)CCN2>>CSC1=NC=CC(=N1)N1CCN2C1=CC(=CC2=O)C2=CC=CC=C2
O=c1cc(-c2ccccc2)cc2n1CCCN2[c:7]1[cH:6][cH:5][n:4][c:3]([S:2][CH3:1])[n:24]1.[NH:8]1[CH2:9][CH2:10][n:11]2[c:12]1[cH:13][c:14](-[c:15]1[cH:16][cH:17][cH:18][cH:19][cH:20]1)[cH:21][c:22]2=[O:23]>>[CH3:1][S:2][c:3]1[n:4][cH:5][cH:6][c:7]([N:8]2[CH2:9][CH2:10][n:11]3[c:12]2[cH:13][c:14](-[c:15]2[cH:16][cH:17][cH:18][cH:19...
CSc1nccc(N2CCCn3c2cc(-c2ccccc2)cc3=O)n1.O=c1cc(-c2ccccc2)cc2n1CCN2
CSc1nccc(N2CCn3c2cc(-c2ccccc2)cc3=O)n1
null
null
C1(=CC=CC=C1)C
Heteroatom Alkylation and Arylation
OtherReaction
e2b33769f44b219d3911e221846a6046a9fb7a29efe4d8dae8fcb782a638ee06
b1a89fc7d17633bbf5e21d37b95beb5c9a8a0ceb9b07eaaec09195f87467174d
O=c1cc(-c2ccccc2)cc2n1CCN2c1ccncn1
O=c1:c:c(-c2:c:c:c:c:c:2):c:c2:n:1-C-C-C-N-2-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](-[#16:4]):[#7;a:5]:[c:6]:[c:7]:1.[c:8]:[c:9]1:[#7;a:10](:[c:11])-[C:12]-[C:13]-[NH;D2;+0:14]-1>>[#16:4]-[c:3]1:[#7;a:2]:[c;H0;D3;+0:1](-[N;H0;D3;+0:14]2-[C:13]-[C:12]-[#7;a:10](:[c:11]):[c:9]-2:[c:8]):[c:7]:[c:6]:[#7;a:5]:1
null
[]
null
null
null
null
Following the procedure described for the synthesis of 1-(2-methylsulfanyl-pyrimidin -4-yl)-8-phenyl-1,2,3,4-tetrahydro-pyrido[1,2-a]pyrimidin-6-one, but using 7-phenyl-2,3-dihydro-1H-imidazo[1,2-a]pyridin-5-one (1 g, 4.7 mmol), sodium tert-butoxide (1.26 g, 13.16 mmol), BINAP (0.43 g, 0.7 mmol), Pd (OAc)2 (0.16 g, 0.7...
10.6084/m9.figshare.5104873.v1
null
Secondary amine.Tertiary amine
Tertiary amine
c1ccccc1.c1ccn2c(c1)NCCC2.c1cncnc1.c1ccn2c(c1)NCC2
c1cncnc1.c1ccn2c(c1)NCC2
c1cncnc1.c1ccn2c(c1)NCC2.c1ccccc1
HO-
C1(=CC=CC=C1)C
null
null
CSc1nccc(N2CCCn3c2cc(-c2ccccc2)cc3=O)n1.O=c1cc(-c2ccccc2)cc2n1CCN2>C1(=CC=CC=C1)C>CSc1nccc(N2CCn3c2cc(-c2ccccc2)cc3=O)n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b0cd299ad92a4b7097196a47ab40341a
Clc1ccnc(Cl)n1.O=c1cc(-c2ccccc2)cc2n1CCN2>>O=c1cc(-c2ccccc2)cc2n1CCN2c1cncc(Cl)n1
CSC1=NC=CC(=N1)N1CCN2C1=CC(=CC2=O)C2=CC=CC=C2.ClC1=NC(=CC=N1)Cl.C1(=CC=CC=C1)C=1C=C2N(C(C1)=O)CCN2>>ClC1=CN=CC(=N1)N1CCN2C1=CC(=CC2=O)C2=CC=CC=C2
Cl[c:17]1[n:19][cH:18][cH:20][c:21]([Cl:22])[n:23]1.[O:1]=[c:2]1[cH:3][c:4](-[c:5]2[cH:6][cH:7][cH:8][cH:9][cH:10]2)[cH:11][c:12]2[n:13]1[CH2:14][CH2:15][NH:16]2>>[O:1]=[c:2]1[cH:3][c:4](-[c:5]2[cH:6][cH:7][cH:8][cH:9][cH:10]2)[cH:11][c:12]2[n:13]1[CH2:14][CH2:15][N:16]2[c:17]1[cH:18][n:19][cH:20][c:21]([Cl:22])[n:23]1
Clc1ccnc(Cl)n1.O=c1cc(-c2ccccc2)cc2n1CCN2
O=c1cc(-c2ccccc2)cc2n1CCN2c1cncc(Cl)n1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
8a5eb1ce9b1cd9e06dadef4c5b5ef114ec706cec868b5a6d8efbea66303ae584
b6b8e2cdb45054a35f5e8157d624f852c0601a09401556706e166b19536eb7a7
O=c1cc(-c2ccccc2)cc2n1CCN2c1cnccn1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](-[Cl;D1;H0:4]):[cH;D2;+0:5]:[cH;D2;+0:6]:[n;H0;D2;+0:7]:1.[c:8]:[c:9]1:[#7;a:10](:[c:11])-[C:12]-[C:13]-[NH;D2;+0:14]-1>>[Cl;D1;H0:4]-[c:3]1:[#7;a:2]:[c;H0;D3;+0:1](-[N;H0;D3;+0:14]2-[C:13]-[C:12]-[#7;a:10](:[c:11]):[c:9]-2:[c:8]):[cH;D2;+0:6]:[n;H0;D2;+0:7]:[cH;D2;+0:5]:1
null
[]
null
null
null
null
Following the procedure described in the synthesis of 1-(2-methylsulfanyl-pyrimidin -4-yl)-7-phenyl-2,3-dihydro-1H-imidazo[1,2-a]pyridin-5-one, but using 2,6-dichloropyrimidine as the coupling component, 7-phenyl-2,3-dihydro-1H-imidazo[1,2-a]pyridin-5-one (0.5 g, 2.4 mmol) was converted into the title product as a pale...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Secondary amine
Tertiary amine
c1cncnc1.c1ccn2c(c1)NCC2
c1ccn2c(c1)NCC2.c1cnccn1
c1ccccc1.c1ccn2c(c1)NCC2.c1cnccn1
HCl
null
null
null
Clc1ccnc(Cl)n1.O=c1cc(-c2ccccc2)cc2n1CCN2>>O=c1cc(-c2ccccc2)cc2n1CCN2c1cncc(Cl)n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e7e6c74594c84cb8bade5396c7aa9e05
NCCc1ccccc1Cl.O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccccc2)n1>>O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccccc2Cl)n1
C(CC1=CC=CC=C1)NC1=NC=CC(=N1)N1C=2N(CCC1)C(C=C(C2)C2=CC=CC=C2)=O.ClC1=C(C=CC=C1)CCN>>ClC1=C(C=CC=C1)CCNC1=NC=CC(=N1)N1C=2N(CCC1)C(C=C(C2)C2=CC=CC=C2)=O
[NH2:23][CH2:24][CH2:25][c:26]1[cH:27][cH:28][cH:29][cH:30][c:31]1[Cl:32].c1ccc(CCN[c:22]2[n:21][cH:20][cH:19][c:18]([N:17]3[c:12]4[cH:11][c:4](-[c:5]5[cH:6][cH:7][cH:8][cH:9][cH:10]5)[cH:3][c:2](=[O:1])[n:13]4[CH2:14][CH2:15][CH2:16]3)[n:33]2)cc1>>[O:1]=[c:2]1[cH:3][c:4](-[c:5]2[cH:6][cH:7][cH:8][cH:9][cH:10]2)[cH:11]...
NCCc1ccccc1Cl.O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccccc2)n1
O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccccc2Cl)n1
null
null
null
Heteroatom Alkylation and Arylation
Chlorination
2869fd0770195ad0aa4896cefd4a8639a5d167b5b710a52d5851c30184610240
56c236df53b2bac39dd5009577ad83355284f0665c6e7906bf125e9599e48527
O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccccc2)n1
[C:1]-[C:2]-[NH2;D1;+0:3].[c:4]:[#7;a:5]:[c;H0;D3;+0:6](-N-C-C-c1:c:c:c:c:c:1):[#7;a:7]:[c:8]>>[C:1]-[C:2]-[NH;D2;+0:3]-[c;H0;D3;+0:6](:[#7;a:7]:[c:8]):[#7;a:5]:[c:4]
null
[]
null
null
null
null
Followed the same procedure described for the synthesis of 1-(2-phenethylamino-pyrimidin-4-yl)-8-phenyl-1,2,3,4-tetrahydro -pyrido[1,2-a]pyrimidin-6-one, the sulfoxide (0.22 g, 0.6 mmol) was displaced with 2-(2-chlorophenyl)ethylamine (0.25 mL, 1.8 mmol) to give the title compound as a yellow solid. MS m/e 458 (M+H)+. ...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Secondary amine
Secondary amine
c1ccccc1.c1cncnc1
c1cncnc1
c1ccccc1.c1ccn2c(c1)NCCC2.c1cncnc1.c1ccccc1
Other
null
null
null
NCCc1ccccc1Cl.O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccccc2)n1>>O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccccc2Cl)n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0c92194a3bb043a390e449a7f49338dd
NCCc1c(Cl)cccc1Cl.O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccccc2)n1>>O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2c(Cl)cccc2Cl)n1
C(CC1=CC=CC=C1)NC1=NC=CC(=N1)N1C=2N(CCC1)C(C=C(C2)C2=CC=CC=C2)=O.ClC1=C(C(=CC=C1)Cl)CCN>>ClC1=C(C(=CC=C1)Cl)CCNC1=NC=CC(=N1)N1C=2N(CCC1)C(C=C(C2)C2=CC=CC=C2)=O
NCC[c:26]1[c:27]([Cl:28])[cH:29][cH:30][cH:31][c:32]1[Cl:33].c1ccc([CH2:25][CH2:24][NH:23][c:22]2[n:21][cH:20][cH:19][c:18]([N:17]3[c:12]4[cH:11][c:4](-[c:5]5[cH:6][cH:7][cH:8][cH:9][cH:10]5)[cH:3][c:2](=[O:1])[n:13]4[CH2:14][CH2:15][CH2:16]3)[n:34]2)cc1>>[O:1]=[c:2]1[cH:3][c:4](-[c:5]2[cH:6][cH:7][cH:8][cH:9][cH:10]2)...
NCCc1c(Cl)cccc1Cl.O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccccc2)n1
O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2c(Cl)cccc2Cl)n1
null
null
null
C-C Coupling
OtherReaction
4be5bc10b11730334b74b64301940b91623d7d2ecad7d43a0b952417d4e4e375
b4142dbc8aebf8ea5ecf50af61f2215c729ea5a2dcf1f9e7fd52e13ad01c499d
O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccccc2)n1
N-C-C-[c;H0;D3;+0:1](:[c:2](-[Cl;D1;H0:3]):[c:4]):[c:5](-[Cl;D1;H0:6]):[c:7].[#7:8]-[C:9]-[CH2;D2;+0:10]-c1:c:c:c:c:c:1>>[#7:8]-[C:9]-[CH2;D2;+0:10]-[c;H0;D3;+0:1](:[c:2](-[Cl;D1;H0:3]):[c:4]):[c:5](-[Cl;D1;H0:6]):[c:7]
null
[]
null
null
null
null
Followed the same procedure described for the synthesis of 1-(2-phenethylamino-pyrimidin-4-yl)-8-phenyl-1,2,3,4-tetrahydro -pyrido[1,2-a]pyrimidin-6-one, the sulfoxide (0.1 g, 0.27 mmol) was displaced with 2-(2,6-dichlorophenyl)ethylamine (0.16 g, 0.82 mmol) to give the title compound as a yellow solid. MS m/e 492 (M+H...
10.6084/m9.figshare.5104873.v1
null
Primary amine
null
c1ccccc1.c1ccccc1
c1ccccc1
c1ccccc1.c1ccn2c(c1)NCCC2.c1cncnc1.c1ccccc1
Other
null
null
null
NCCc1c(Cl)cccc1Cl.O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccccc2)n1>>O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2c(Cl)cccc2Cl)n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-04477d4233fe48f89bed229349edc82b
NCCc1ccc(Cl)cc1Cl.O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccccc2)n1>>O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccc(Cl)cc2Cl)n1
C(CC1=CC=CC=C1)NC1=NC=CC(=N1)N1C=2N(CCC1)C(C=C(C2)C2=CC=CC=C2)=O.ClC1=C(C=CC(=C1)Cl)CCN>>ClC1=C(C=CC(=C1)Cl)CCNC1=NC=CC(=N1)N1C=2N(CCC1)C(C=C(C2)C2=CC=CC=C2)=O
NCC[c:26]1[cH:27][cH:28][c:29]([Cl:30])[cH:31][c:32]1[Cl:33].c1ccc([CH2:25][CH2:24][NH:23][c:22]2[n:21][cH:20][cH:19][c:18]([N:17]3[c:12]4[cH:11][c:4](-[c:5]5[cH:6][cH:7][cH:8][cH:9][cH:10]5)[cH:3][c:2](=[O:1])[n:13]4[CH2:14][CH2:15][CH2:16]3)[n:34]2)cc1>>[O:1]=[c:2]1[cH:3][c:4](-[c:5]2[cH:6][cH:7][cH:8][cH:9][cH:10]2)...
NCCc1ccc(Cl)cc1Cl.O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccccc2)n1
O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccc(Cl)cc2Cl)n1
null
null
null
C-C Coupling
OtherReaction
4be5bc10b11730334b74b64301940b91623d7d2ecad7d43a0b952417d4e4e375
b4142dbc8aebf8ea5ecf50af61f2215c729ea5a2dcf1f9e7fd52e13ad01c499d
O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccccc2)n1
N-C-C-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[Cl;D1;H0:5]):[c:6].[#7:7]-[C:8]-[CH2;D2;+0:9]-c1:c:c:c:c:c:1>>[#7:7]-[C:8]-[CH2;D2;+0:9]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[Cl;D1;H0:5]):[c:6]
null
[]
null
null
null
null
Followed the same procedure in the synthesis of 1-(2-phenethylamino-pyrimidin-4-yl)-8-phenyl-1,2,3,4-tetrahydro-pyrido[1,2-a]pyrimidin-6-one, the sulfoxide (0.11 g, 0.3 mmol) was displaced with 2-(2,4-dichlorophenyl)ethylamine (0.14 mL, 0.9 mmol) to give the title compound as a yellow solid. MS m/e 492 (M+H)+. Conditio...
10.6084/m9.figshare.5104873.v1
null
Primary amine
null
c1ccccc1.c1ccccc1
c1ccccc1
c1ccccc1.c1ccn2c(c1)NCCC2.c1cncnc1.c1ccccc1
Other
null
null
null
NCCc1ccc(Cl)cc1Cl.O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccccc2)n1>>O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccc(Cl)cc2Cl)n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ad8f2b2f8d6f40b8b539a6bde61a85d7
CC(N)Cc1cccc(CO)c1.O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccccc2)n1>>CC(Cc1cccc(CO)c1)Nc1nccc(N2CCCn3c2cc(-c2ccccc2)cc3=O)n1
C(CC1=CC=CC=C1)NC1=NC=CC(=N1)N1C=2N(CCC1)C(C=C(C2)C2=CC=CC=C2)=O.NC(CC=1C=C(C=CC1)CO)C>>OCC=1C=C(C=CC1)CC(C)NC1=NC=CC(=N1)N1C=2N(CCC1)C(C=C(C2)C2=CC=CC=C2)=O
[CH3:1][CH:2]([CH2:3][c:4]1[cH:5][cH:6][cH:7][c:8]([CH2:9][OH:10])[cH:11]1)[NH2:12].c1ccc(CCN[c:13]2[n:14][cH:15][cH:16][c:17]([N:18]3[CH2:19][CH2:20][CH2:21][n:22]4[c:23]3[cH:24][c:25](-[c:26]3[cH:27][cH:28][cH:29][cH:30][cH:31]3)[cH:32][c:33]4=[O:34])[n:35]2)cc1>>[CH3:1][CH:2]([CH2:3][c:4]1[cH:5][cH:6][cH:7][c:8]([CH...
CC(N)Cc1cccc(CO)c1.O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccccc2)n1
CC(Cc1cccc(CO)c1)Nc1nccc(N2CCCn3c2cc(-c2ccccc2)cc3=O)n1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
2869fd0770195ad0aa4896cefd4a8639a5d167b5b710a52d5851c30184610240
56c236df53b2bac39dd5009577ad83355284f0665c6e7906bf125e9599e48527
O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccccc2)n1
[C:1]-[C:2](-[C;D1;H3:3])-[NH2;D1;+0:4].[c:5]:[#7;a:6]:[c;H0;D3;+0:7](-N-C-C-c1:c:c:c:c:c:1):[#7;a:8]:[c:9]>>[C:1]-[C:2](-[C;D1;H3:3])-[NH;D2;+0:4]-[c;H0;D3;+0:7](:[#7;a:6]:[c:5]):[#7;a:8]:[c:9]
null
[]
null
null
null
null
Following the same procedure described for the synthesis of 1-(2-phenethylamino-pyrimidin-4-yl)-8-phenyl -1,2,3,4-tetrahydro-pyrido[1,2-a]pyrimidin-6-one, the sulfoxide (0.29 g, 0.83 mmol) was displaced with [3-(2-amino-propyl)-phenyl]-methanol (0.3 g, 1.66 mmol) to give the title compound as a light yellow solid. MS m...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Secondary amine
Secondary amine
c1ccccc1.c1cncnc1
c1cncnc1
c1ccccc1.c1cncnc1.c1ccn2c(c1)NCCC2.c1ccccc1
Other
null
null
null
CC(N)Cc1cccc(CO)c1.O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccccc2)n1>>CC(Cc1cccc(CO)c1)Nc1nccc(N2CCCn3c2cc(-c2ccccc2)cc3=O)n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b2f3937799494752b8fbf7e0af1f7829
NCCc1ccccc1.O=c1cc(-c2ccccc2)cc2n1CCCN2c1cc(Cl)ncn1>>O=c1cc(-c2ccccc2)cc2n1CCCN2c1cc(NCCc2ccccc2)ncn1
ClC1=CC(=NC=N1)N1C=2N(CCC1)C(C=C(C2)C2=CC=CC=C2)=O.C(=O)([O-])[O-].[K+].[K+].C(CC1=CC=CC=C1)N>>C(CC1=CC=CC=C1)NC1=CC(=NC=N1)N1C=2N(CCC1)C(C=C(C2)C2=CC=CC=C2)=O
[NH2:21][CH2:22][CH2:23][c:24]1[cH:25][cH:26][cH:27][cH:28][cH:29]1.Cl[c:20]1[cH:19][c:18]([N:17]2[c:12]3[cH:11][c:4](-[c:5]4[cH:6][cH:7][cH:8][cH:9][cH:10]4)[cH:3][c:2](=[O:1])[n:13]3[CH2:14][CH2:15][CH2:16]2)[n:32][cH:31][n:30]1>>[O:1]=[c:2]1[cH:3][c:4](-[c:5]2[cH:6][cH:7][cH:8][cH:9][cH:10]2)[cH:11][c:12]2[n:13]1[CH...
NCCc1ccccc1.O=c1cc(-c2ccccc2)cc2n1CCCN2c1cc(Cl)ncn1
O=c1cc(-c2ccccc2)cc2n1CCCN2c1cc(NCCc2ccccc2)ncn1
null
null
O.CN(C)C=O.CCOC(=O)C
Heteroatom Alkylation and Arylation
N-arylation (Buchwald-Hartwig/Ullmann-Goldberg)
c38b7155556ff28144ae37859ff6668b20d59da60c705d26b158542b6d8385da
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
O=c1cc(-c2ccccc2)cc2n1CCCN2c1cc(NCCc2ccccc2)ncn1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](-[#7:6]):[c:7]:1.[C:8]-[C:9]-[NH2;D1;+0:10]>>[#7:6]-[c:5]1:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:10]-[C:9]-[C:8]):[c:7]:1
null
[]
null
null
null
null
To a stirred mixture of 1-(6-chloro-pyrimidin-4-yl)-8-phenyl -1,2,3,4-tetrahydro-pyrido[1,2-a]pyrimidin-6-one (0.158 mg, 0.47 mmol) and excess of K2CO3 in DMF (3 mL) was added phenethylamine (0.15 mL, 1.2 mmol). The overall reaction vessel was irradiated under microwave conditions at 150° C. for 10 min. After diluted w...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1cncnc1
c1cncnc1
c1ccccc1.c1ccn2c(c1)NCCC2.c1cncnc1.c1ccccc1
HCl
O.CN(C)C=O.CCOC(=O)C
null
null
NCCc1ccccc1.O=c1cc(-c2ccccc2)cc2n1CCCN2c1cc(Cl)ncn1>O.CN(C)C=O.CCOC(=O)C>O=c1cc(-c2ccccc2)cc2n1CCCN2c1cc(NCCc2ccccc2)ncn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-cb6bf0074c9b43fd9e0c98dcafb44ec9
NCCc1ccccc1Cl.O=c1cc(-c2ccccc2)cc2n1CCCN2c1cc(Cl)ncn1>>O=c1cc(-c2ccccc2)cc2n1CCCN2c1cc(NCCc2ccccc2Cl)ncn1
C(CC1=CC=CC=C1)NC1=NC=CC(=N1)N1C=2N(CCC1)C(C=C(C2)C2=CC=CC=C2)=O.ClC1=CC(=NC=N1)N1C=2N(CCC1)C(C=C(C2)C2=CC=CC=C2)=O.ClC1=C(C=CC=C1)CCN>>ClC1=C(C=CC=C1)CCNC1=CC(=NC=N1)N1C=2N(CCC1)C(C=C(C2)C2=CC=CC=C2)=O
[NH2:21][CH2:22][CH2:23][c:24]1[cH:25][cH:26][cH:27][cH:28][c:29]1[Cl:30].Cl[c:20]1[cH:19][c:18]([N:17]2[c:12]3[cH:11][c:4](-[c:5]4[cH:6][cH:7][cH:8][cH:9][cH:10]4)[cH:3][c:2](=[O:1])[n:13]3[CH2:14][CH2:15][CH2:16]2)[n:33][cH:32][n:31]1>>[O:1]=[c:2]1[cH:3][c:4](-[c:5]2[cH:6][cH:7][cH:8][cH:9][cH:10]2)[cH:11][c:12]2[n:1...
NCCc1ccccc1Cl.O=c1cc(-c2ccccc2)cc2n1CCCN2c1cc(Cl)ncn1
O=c1cc(-c2ccccc2)cc2n1CCCN2c1cc(NCCc2ccccc2Cl)ncn1
null
null
null
Heteroatom Alkylation and Arylation
N-arylation (Buchwald-Hartwig/Ullmann-Goldberg)
c38b7155556ff28144ae37859ff6668b20d59da60c705d26b158542b6d8385da
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
O=c1cc(-c2ccccc2)cc2n1CCCN2c1cc(NCCc2ccccc2)ncn1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](-[#7:6]):[c:7]:1.[C:8]-[C:9]-[NH2;D1;+0:10]>>[#7:6]-[c:5]1:[#7;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:10]-[C:9]-[C:8]):[c:7]:1
null
[]
null
null
null
null
Followed the same procedure described for the synthesis of 1-(2-phenethylamino-pyrimidin-4-yl)-8-phenyl-1,2,3,4-tetrahydro -pyrido[1,2-a]pyrimidin-6-one, 1-(6-chloro-pyrimidin-4-yl)-8-phenyl-1,2,3,4-tetrahydro -pyrido[1,2-a]pyrimidin-6-one (0.136 g, 0.40 mmol) was reacted with 2-(2-chlorophenyl)ethylamine (0.17 mL, 1.2...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1cncnc1
c1cncnc1
c1ccccc1.c1ccn2c(c1)NCCC2.c1cncnc1.c1ccccc1
HCl
null
null
null
NCCc1ccccc1Cl.O=c1cc(-c2ccccc2)cc2n1CCCN2c1cc(Cl)ncn1>>O=c1cc(-c2ccccc2)cc2n1CCCN2c1cc(NCCc2ccccc2Cl)ncn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-34f352eead4448779d7bf3a6aa2543d9
CC(N)Cc1cccc(CO)c1.O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccccc2)n1>>CC(Cc1cccc(CO)c1)Nc1nccc(N2CCn3c2cc(-c2ccccc2)cc3=O)n1
C(CC1=CC=CC=C1)NC1=NC=CC(=N1)N1C=2N(CCC1)C(C=C(C2)C2=CC=CC=C2)=O.NC(CC=1C=C(C=CC1)CO)C>>OCC=1C=C(C=CC1)CC(C)NC1=NC=CC(=N1)N1CCN2C1=CC(=CC2=O)C2=CC=CC=C2
[CH3:1][CH:2]([CH2:3][c:4]1[cH:5][cH:6][cH:7][c:8]([CH2:9][OH:10])[cH:11]1)[NH2:12].c1ccc(CCN[c:13]2[n:14][cH:15][cH:16][c:17]([N:18]3C[CH2:19][CH2:20][n:21]4[c:22]3[cH:23][c:24](-[c:25]3[cH:26][cH:27][cH:28][cH:29][cH:30]3)[cH:31][c:32]4=[O:33])[n:34]2)cc1>>[CH3:1][CH:2]([CH2:3][c:4]1[cH:5][cH:6][cH:7][c:8]([CH2:9][OH...
CC(N)Cc1cccc(CO)c1.O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccccc2)n1
CC(Cc1cccc(CO)c1)Nc1nccc(N2CCn3c2cc(-c2ccccc2)cc3=O)n1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
007c6555f8bdc87d89d912e2e910a62cdfe7700b1bcfac6f6083df140cad2f82
fb80d3c6b41d3e084e190e67a9fe6319222a14054de6c86adc01f47a0c5fc4e1
O=c1cc(-c2ccccc2)cc2n1CCN2c1ccnc(NCCc2ccccc2)n1
[C:1]-[C:2](-[C;D1;H3:3])-[NH2;D1;+0:4].[c:5]:[c:6]1:[#7;a:7](:[c:8])-[C:9]-[CH2;D2;+0:10]-C-[N;H0;D3;+0:11]-1-[c:12]1:[#7;a:13]:[c;H0;D3;+0:14](-N-C-C-c2:c:c:c:c:c:2):[#7;a:15]:[c:16]:[c:17]:1>>[C:1]-[C:2](-[C;D1;H3:3])-[NH;D2;+0:4]-[c;H0;D3;+0:14]1:[#7;a:15]:[c:16]:[c:17]:[c:12](-[N;H0;D3;+0:11]2-[CH2;D2;+0:10]-[C:9]...
null
[]
null
null
null
null
Following the same procedure described for the synthesis of 1-(2-phenethylamino-pyrimidin-4-yl)-8-phenyl-1,2,3,4-tetrahydro-pyrido[1,2-a]pyrimidin-6-one, the sulfoxide/sulfone (0.4 g) was displaced with [3-(2-amino-propyl)-phenyl]-methanol (1.2 eq) to give the title compound as a light yellow solid. MS m/e 454 (M+H)+. ...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Secondary amine.Tertiary amine
Secondary amine.Tertiary amine
c1ccccc1.c1cncnc1.c1ccn2c(c1)NCCC2
c1cncnc1.c1ccn2c(c1)NCC2
c1ccccc1.c1cncnc1.c1ccn2c(c1)NCC2.c1ccccc1
Other
null
null
null
CC(N)Cc1cccc(CO)c1.O=c1cc(-c2ccccc2)cc2n1CCCN2c1ccnc(NCCc2ccccc2)n1>>CC(Cc1cccc(CO)c1)Nc1nccc(N2CCn3c2cc(-c2ccccc2)cc3=O)n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ba1c8c7437684ce38dd842cb5b96d860
NCCc1ccccc1.O=c1cc(-c2ccccc2)cc2n1CCN2c1cncc(Cl)n1>>O=c1cc(-c2ccccc2)cc2n1CCN2c1cncc(NCCc2ccccc2)n1
C(CC1=CC=CC=C1)N.ClC1=CN=CC(=N1)N1CCN2C1=CC(=CC2=O)C2=CC=CC=C2.CC(C)([O-])C.[Na+].C=1C=CC(=CC1)P(C=2C=CC=CC2)C3=CC=C4C=CC=CC4=C3C5=C6C=CC=CC6=CC=C5P(C=7C=CC=CC7)C=8C=CC=CC8>>C(CC1=CC=CC=C1)NC1=CN=CC(=N1)N1CCN2C1=CC(=CC2=O)C2=CC=CC=C2
[NH2:22][CH2:23][CH2:24][c:25]1[cH:26][cH:27][cH:28][cH:29][cH:30]1.Cl[c:21]1[cH:20][n:19][cH:18][c:17]([N:16]2[c:12]3[cH:11][c:4](-[c:5]4[cH:6][cH:7][cH:8][cH:9][cH:10]4)[cH:3][c:2](=[O:1])[n:13]3[CH2:14][CH2:15]2)[n:31]1>>[O:1]=[c:2]1[cH:3][c:4](-[c:5]2[cH:6][cH:7][cH:8][cH:9][cH:10]2)[cH:11][c:12]2[n:13]1[CH2:14][CH...
NCCc1ccccc1.O=c1cc(-c2ccccc2)cc2n1CCN2c1cncc(Cl)n1
O=c1cc(-c2ccccc2)cc2n1CCN2c1cncc(NCCc2ccccc2)n1
null
null
C1(=CC=CC=C1)C
Heteroatom Alkylation and Arylation
N-arylation (Buchwald-Hartwig/Ullmann-Goldberg)
d8d76a4347a32a5acf79894f48887cf8d745ba4ca5f91e54084ebdbe25f43c75
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
O=c1cc(-c2ccccc2)cc2n1CCN2c1cncc(NCCc2ccccc2)n1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5]:[c:6]:1.[C:7]-[C:8]-[NH2;D1;+0:9]>>[C:7]-[C:8]-[NH;D2;+0:9]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#7;a:5]:[c:6]:1
null
[]
70
CELSIUS
null
null
To a mixture of 1-(6-chloro-pyrazin-2-yl)-7-phenyl-2,3-dihydro-1H-imidazo[1,2-a]pyridin-5-one (85 mg, 0.26 mmol), sodium tert-butoxide (70 mg, 2.8 eq), BINAP (24 mg, 15% eq), and Pd (OAc)2 (9 mg, 15% eq) was added toluene (5 mL) and phenethylamine (39 μL, 1.2 eq). After purged with N2 for 10 min, the overall mixture wa...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1cnccn1
c1cnccn1
c1ccccc1.c1ccn2c(c1)NCC2.c1cnccn1.c1ccccc1
HCl
C1(=CC=CC=C1)C
70
null
NCCc1ccccc1.O=c1cc(-c2ccccc2)cc2n1CCN2c1cncc(Cl)n1>C1(=CC=CC=C1)C>O=c1cc(-c2ccccc2)cc2n1CCN2c1cncc(NCCc2ccccc2)n1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ebeeb039964a4f5b90012c8ce5c1b9a9
CCOC(=O)CBr.c1ccc(CNNCc2ccccc2)cc1>>NCC(=O)O.c1ccc(CNNCc2ccccc2)cc1
BrCC(=O)OCC.C(C1=CC=CC=C1)NNCC1=CC=CC=C1.C1CCOC1.BrCC(=O)OCC>>NCC(=O)O.C(C1=CC=CC=C1)NNCC1=CC=CC=C1
CC[O:5][C:3]([CH2:2]Br)=[O:4].[NH:1]([CH2:10][c:9]1[cH:8][cH:7][cH:6][cH:21][cH:20]1)[NH:12][CH2:13][c:14]1[cH:15][cH:16][cH:17][cH:18][cH:19]1>>[NH2:1][CH2:2][C:3](=[O:4])[OH:5].[cH:6]1[cH:7][cH:8][c:9]([CH2:10][NH:11][NH:12][CH2:13][c:14]2[cH:15][cH:16][cH:17][cH:18][cH:19]2)[cH:20][cH:21]1
CCOC(=O)CBr.c1ccc(CNNCc2ccccc2)cc1
NCC(=O)O.c1ccc(CNNCc2ccccc2)cc1
null
CCCC[N+](CCCC)(CCCC)CCCC.[I-]
CCN(CC)CC
Heteroatom Alkylation and Arylation
OtherReaction
75da99c5c8d92cc69676755c7566deba3a404ac4d1c9feac0426623d6ce52991
da708edba4837b1998751e9cba8b74e9330f39096dc25117914a4af61948a33f
c1ccc(CNNCc2ccccc2)cc1
Br-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[O;H0;D2;+0:4]-C-C.[c:5]-[C:6]-[NH;D2;+0:7]-[NH;D2;+0:8]-[CH2;D2;+0:9]-[c:10](:[c:11]):[c:12]>>[NH2;D1;+0:8]-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:4].[c:5]-[C:6]-[NH;D2;+0:7]-[#7:13]-[CH2;D2;+0:9]-[c:10](:[c:11]):[c:12]
97
[{"value": 97.0, "product": "NCC(=O)O.C(C1=CC=CC=C1)NNCC1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}]
60
CELSIUS
7
HOUR
To a solution of dibenzylhydrazine (5.30 g, 25.0 mmol) and THF (50 mL) and TBAI (0.46 g, 1.25 mmol) was added BrCH2CO2Et (2.64 mL, 23.8 mmol) and Et3N (3.32 mL, 23.8 mmol). The reaction mixture was stirred at 60° C. for 7 hours, an additional 0.3 eq. of base and electrophile were added (BrCH2CO2Et, 0.83 mL, 7.5 mmol an...
10.6084/m9.figshare.5104873.v1
null
Hydrazine.Primary halide.Ester
Hydrazine.Carboxylic acid.Primary amine
null
null
c1ccccc1.c1ccccc1
HBr
CCCC[N+](CCCC)(CCCC)CCCC.[I-].CCN(CC)CC
60
7
CCOC(=O)CBr.c1ccc(CNNCc2ccccc2)cc1>CCCC[N+](CCCC)(CCCC)CCCC.[I-].CCN(CC)CC>NCC(=O)O.c1ccc(CNNCc2ccccc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0af8c32461614a67a44ada3a3898c093
CCOC(=O)c1sc(Cl)nc1-c1ccccc1.COc1cc2nc[nH]c2cc1OC>>CCOC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1
O.COC1=CC2=C(N=CN2)C=C1OC.[H-].[Na+].C(C)OC(=O)C1=C(N=C(S1)Cl)C1=CC=CC=C1>>C(C)OC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC=CC=C2
Cl[c:8]1[s:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[c:23](-[c:24]2[cH:25][cH:26][cH:27][cH:28][cH:29]2)[n:22]1.[nH:9]1[cH:10][n:11][c:12]2[cH:13][c:14]([O:15][CH3:16])[c:17]([O:18][CH3:19])[cH:20][c:21]12>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[s:7][c:8](-[n:9]2[cH:10][n:11][c:12]3[cH:13][c:14]([O:15][CH3:16])[c:17]([...
CCOC(=O)c1sc(Cl)nc1-c1ccccc1.COc1cc2nc[nH]c2cc1OC
CCOC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1
null
null
CN1CCCC1=O
Heteroatom Alkylation and Arylation
OtherReaction
b38f76237cdec2baf41c9411839797fed979828e4dd9354fb2aa8a56efaef6ba
e3660767655c50df0f92afc78c794dd2af7cf646bf1430960eafd30c23bf3fa7
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Cl-[c;H0;D3;+0:1]1:[#16;a:2]:[c:3](-[C:4](-[#8:5])=[O;D1;H0:6]):[c:7]:[#7;a:8]:1.[c:9]:[c:10]1:[#7;a:11]:[c:12]:[nH;D2;+0:13]:[c:14]:1:[c:15]>>[#8:5]-[C:4](=[O;D1;H0:6])-[c:3]1:[#16;a:2]:[c;H0;D3;+0:1](-[n;H0;D3;+0:13]2:[c:12]:[#7;a:11]:[c:10](:[c:9]):[c:14]:2:[c:15]):[#7;a:8]:[c:7]:1
84
[{"value": 84.0, "product": "C(C)OC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC=CC=C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 83.6, "product": "C(C)OC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC=CC=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
20
MINUTE
5,6-Dimethoxybenzimidazole (470 mg, 2.64 mmol) was added to a suspension of NaH (60% in mineral oil, 112 mg, 2.8 mmol) in NMP (5 ml) at <5° C. The mixture was stirred for 20 min, then a solution of 2-chloro-4-phenylthiazole-5-carboxylic acid ethyl ester (589 mg, 2.2 mmol) in NMP (1.5 ml) was added over 2-3 min. The mix...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1cscn1.c1ccc2[nH]cnc2c1
c1cscn1.c1ccc2[nH]cnc2c1
c1cscn1.c1ccc2[nH]cnc2c1.c1ccccc1
HCl
CN1CCCC1=O
null
0.333333
CCOC(=O)c1sc(Cl)nc1-c1ccccc1.COc1cc2nc[nH]c2cc1OC>CN1CCCC1=O>CCOC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c9ff6485c25c4a798f1ff4bd86c8e00b
CCOC(=O)c1sc(Cl)nc1-c1ccccc1.c1ccc2[nH]cnc2c1>>CCOC(=O)c1sc(-n2cnc3ccccc32)nc1-c1ccccc1
O.C(C)OC(=O)C1=C(N=C(S1)Cl)C1=CC=CC=C1.N1=CNC2=C1C=CC=C2.[Li]N([Si](C)(C)C)[Si](C)(C)C>>C(C)OC(=O)C1=C(N=C(S1)N1C=NC2=C1C=CC=C2)C2=CC=CC=C2
Cl[c:8]1[s:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[c:19](-[c:20]2[cH:21][cH:22][cH:23][cH:24][cH:25]2)[n:18]1.[nH:9]1[cH:10][n:11][c:12]2[cH:13][cH:14][cH:15][cH:16][c:17]12>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[s:7][c:8](-[n:9]2[cH:10][n:11][c:12]3[cH:13][cH:14][cH:15][cH:16][c:17]23)[n:18][c:19]1-[c:20]1[cH:21][c...
CCOC(=O)c1sc(Cl)nc1-c1ccccc1.c1ccc2[nH]cnc2c1
CCOC(=O)c1sc(-n2cnc3ccccc32)nc1-c1ccccc1
null
null
O1CCCC1
Heteroatom Alkylation and Arylation
OtherReaction
b38f76237cdec2baf41c9411839797fed979828e4dd9354fb2aa8a56efaef6ba
e3660767655c50df0f92afc78c794dd2af7cf646bf1430960eafd30c23bf3fa7
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Cl-[c;H0;D3;+0:1]1:[#16;a:2]:[c:3](-[C:4](-[#8:5])=[O;D1;H0:6]):[c:7]:[#7;a:8]:1.[c:9]:[c:10]1:[#7;a:11]:[c:12]:[nH;D2;+0:13]:[c:14]:1:[c:15]>>[#8:5]-[C:4](=[O;D1;H0:6])-[c:3]1:[#16;a:2]:[c;H0;D3;+0:1](-[n;H0;D3;+0:13]2:[c:12]:[#7;a:11]:[c:10](:[c:9]):[c:14]:2:[c:15]):[#7;a:8]:[c:7]:1
61.8
[{"value": 61.0, "product": "C(C)OC(=O)C1=C(N=C(S1)N1C=NC2=C1C=CC=C2)C2=CC=CC=C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 61.8, "product": "C(C)OC(=O)C1=C(N=C(S1)N1C=NC2=C1C=CC=C2)C2=CC=CC=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
120
CELSIUS
null
null
A mixture of 2-chloro-4-phenylthiazole-5-carboxylic acid ethyl ester (134 mg, 0.5 mmol), benzimidazole (Aldrich) (73.8 mg, 0.625 mmol) and LiN(TMS)2 (1N tetrahydrofuran solution, 0.63 ml) in tetrahydrofuran (2 ml) was heated in a micro-wave oven at 120° C. for 30 min. Water (3 ml) was added and the mixture was filtered...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1cscn1.c1ccc2[nH]cnc2c1
c1cscn1.c1ccc2[nH]cnc2c1
c1cscn1.c1ccc2[nH]cnc2c1.c1ccccc1
HCl
O1CCCC1
120
null
CCOC(=O)c1sc(Cl)nc1-c1ccccc1.c1ccc2[nH]cnc2c1>O1CCCC1>CCOC(=O)c1sc(-n2cnc3ccccc32)nc1-c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a21b61bc535644b9b17a1f6bd9ccfbba
O=Cc1sc(Br)nc1Br.[O]=[Mn](=[O])(=[O])[O-]>>O=C(O)c1sc(Br)nc1Br
[Mn](=O)(=O)(=O)[O-].[K+].BrC=1SC(=C(N1)Br)C=O.[Mn](=O)(=O)(=O)[O-].[K+]>>BrC=1SC(=C(N1)Br)C(=O)O
[O:1]=[CH:2][c:4]1[s:5][c:6]([Br:7])[n:8][c:9]1[Br:10].[O]=[Mn](=[O])(=[O])[O-:3]>>[O:1]=[C:2]([OH:3])[c:4]1[s:5][c:6]([Br:7])[n:8][c:9]1[Br:10]
O=Cc1sc(Br)nc1Br.[O]=[Mn](=[O])(=[O])[O-]
O=C(O)c1sc(Br)nc1Br
null
null
O
Acylation
OtherReaction
212580cf94343ba681451fe636f6c4d850d6e10e1bdc7e1852b33ddb4cd6898f
37c4d4a9954dede23d940a212db876610ae18deb2faf143c8b44e17692b9193f
c1cscn1
[Br;D1;H0:1]-[c:2]1:[#7;a:3]:[c:4]:[#16;a:5]:[c:6]:1-[CH;D2;+0:7]=[O;D1;H0:8].[O-;H0;D1:9]-[Mn](=[O])(=[O])=[O]>>[Br;D1;H0:1]-[c:2]1:[#7;a:3]:[c:4]:[#16;a:5]:[c:6]:1-[C;H0;D3;+0:7](=[O;D1;H0:8])-[OH;D1;+0:9]
null
[]
null
null
null
null
Solid potassium permanganate (2.19 g, 13.85 mmol) was added portionwise to a hot suspension of 2,4-dibromo-thiazole-5-carbaldehyde (2.5 g, 9.23 mmol) in water (20 ml). The progress of the reaction was monitored by HPLC. More potassium permanganate was added until all of the aldehyde was consumed. The dark suspension wa...
10.6084/m9.figshare.5104873.v1
null
Aldehyde
Carboxylic acid
null
null
c1cscn1
Other
O
null
null
O=Cc1sc(Br)nc1Br.[O]=[Mn](=[O])(=[O])[O-]>O>O=C(O)c1sc(Br)nc1Br
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6af32ca2635141ed8b014e6444daca2b
O=C(O)c1sc(Br)nc1Br>>COC(=O)c1sc(Br)nc1Br
BrC=1SC(=C(N1)Br)C(=O)O.CN(CCCN=C=NCC)C>>COC(=O)C1=C(N=C(S1)Br)Br
[OH:2][C:3](=[O:4])[c:5]1[s:6][c:7]([Br:8])[n:9][c:10]1[Br:11]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[s:6][c:7]([Br:8])[n:9][c:10]1[Br:11]
O=C(O)c1sc(Br)nc1Br
COC(=O)c1sc(Br)nc1Br
null
null
CO
Miscellaneous
Protection of carboxylic acid
56520e0abb4535dce9a663824ca803b71c2c0dd72dfd246317d953596a987bd2
2ccc7a30191c2c171b49e8a0217bee87430687dd0f567141eca025a75b7e3136
c1cscn1
[#16;a:1]:[c:2](-[C:3](=[O;D1;H0:4])-[OH;D1;+0:5]):[c:6]:[#7;a:7]>>[#16;a:1]:[c:2](-[C:3](=[O;D1;H0:4])-[O;H0;D2;+0:5]-[C;D1;H3:8]):[c:6]:[#7;a:7]
78.6
[{"value": 78.0, "product": "COC(=O)C1=C(N=C(S1)Br)Br", "details": "PERCENTYIELD", "is_desired": false}, {"value": 78.6, "product": "COC(=O)C1=C(N=C(S1)Br)Br", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
A solution of 2,4-dibromo-thiazole-5-carboxylic acid (1.7 g, 5.92 mmol) in methanol (20 ml) was treated with N-(3-dimethylaminopropyl)-N′-ethylcarbodiimide (920 mg, 5.92 mmol). The mixture was stirred at ambient temperature overnight. The solvent was evaporated and water (30 ml) was added. The mixture was then extracte...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Ester
null
null
c1cscn1
Other
CO
null
8
O=C(O)c1sc(Br)nc1Br>CO>COC(=O)c1sc(Br)nc1Br
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-342d8b1c96644769bb9b2301fe33859a
COC(=O)c1sc(Br)nc1Br.COc1cc2nc[nH]c2cc1OC>>COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br
O.COC(=O)C1=C(N=C(S1)Br)Br.COC1=CC2=C(NC=N2)C=C1OC.[H-].[Na+]>>COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br
Br[c:7]1[s:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[c:22]([Br:23])[n:21]1.[nH:8]1[cH:9][n:10][c:11]2[cH:12][c:13]([O:14][CH3:15])[c:16]([O:17][CH3:18])[cH:19][c:20]12>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[s:6][c:7](-[n:8]2[cH:9][n:10][c:11]3[cH:12][c:13]([O:14][CH3:15])[c:16]([O:17][CH3:18])[cH:19][c:20]23)[n:21][c:22]1[Br:23]
COC(=O)c1sc(Br)nc1Br.COc1cc2nc[nH]c2cc1OC
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br
null
null
CN1C(CCC1)=O
Heteroatom Alkylation and Arylation
OtherReaction
b38f76237cdec2baf41c9411839797fed979828e4dd9354fb2aa8a56efaef6ba
e3660767655c50df0f92afc78c794dd2af7cf646bf1430960eafd30c23bf3fa7
c1ccc2c(c1)ncn2-c1nccs1
Br-[c;H0;D3;+0:1]1:[#16;a:2]:[c:3](-[C:4](-[#8:5])=[O;D1;H0:6]):[c:7]:[#7;a:8]:1.[c:9]:[c:10]1:[#7;a:11]:[c:12]:[nH;D2;+0:13]:[c:14]:1:[c:15]>>[#8:5]-[C:4](=[O;D1;H0:6])-[c:3]1:[#16;a:2]:[c;H0;D3;+0:1](-[n;H0;D3;+0:13]2:[c:12]:[#7;a:11]:[c:10](:[c:9]):[c:14]:2:[c:15]):[#7;a:8]:[c:7]:1
73
[{"value": 73.0, "product": "COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br", "details": "PERCENTYIELD", "is_desired": false}, {"value": 71.1, "product": "COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a solution of 5,6-Dimethoxy-1H-benzimidazole (1.0 g, 5.65 mmol) in 1-methyl-2-pyrrolidinone (10 ml) at 0° C. was added NaH (60% dispersion; 339 mg, 8.475 mmol). After gas evolution had stopped, 2,4-Dibromo-thiazole-5-carboxylic acid methyl ester (1.7 g, 5.65 mmol) was added. The resulting solution was stirred at amb...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1cscn1.c1ccc2[nH]cnc2c1
c1cscn1.c1ccc2[nH]cnc2c1
c1cscn1.c1ccc2[nH]cnc2c1
HBr
CN1C(CCC1)=O
null
1
COC(=O)c1sc(Br)nc1Br.COc1cc2nc[nH]c2cc1OC>CN1C(CCC1)=O>COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8df2b2f2ab9843b1ad9a8483dab5bafd
CCOC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1>>COc1cc2ncn(-c3nc(-c4ccccc4)c(C(=O)O)s3)c2cc1OC
C(C)OC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC=CC=C2.[OH-].[Na+].O>>COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=CC=C2)C(=O)O)C=C1OC
CC[O:21][C:19]([c:18]1[c:11](-[c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:25]([O:26][CH3:27])[cH:24][c:23]32)[s:22]1)=[O:20]>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][cH:15][cH:16][cH:17]4)[c:18]([C:19](=[O:...
CCOC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1
COc1cc2ncn(-c3nc(-c4ccccc4)c(C(=O)O)s3)c2cc1OC
null
null
C1CCOC1
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4](:[#16;a:5]):[c:6]:[#7;a:7]>>[#16;a:5]:[c:4](-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]):[c:6]:[#7;a:7]
88
[{"value": 88.0, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=CC=C2)C(=O)O)C=C1OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 86.4, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=CC=C2)C(=O)O)C=C1OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
2-(5,6-Dimethoxybenzoimidazol-1-yl)-4-phenylthiazole-5-carboxylic acid ethyl ester (180 mg, 0.44 mmol) was suspended in THF (4 ml), NaOH (15%, 1.5 ml) and water (2 ml) and the mixture was stirred at 40-50° C. for 3 hrs. After THF was removed, the residue was extracted with ethyl acetate (2×2 mL). The aqueous was then n...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1
Other
C1CCOC1
null
null
CCOC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1>C1CCOC1>COc1cc2ncn(-c3nc(-c4ccccc4)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-bb4775cc5c1145c0a1255bd2f894cd37
CCOC(=O)c1sc(-n2cnc3ccccc32)nc1-c1ccccc1.[NH4+]>>NC(=O)c1sc(-n2cnc3ccccc32)nc1-c1ccccc1
FC(C(=O)O)(F)F.C(C)OC(=O)C1=C(N=C(S1)N1C=NC2=C1C=CC=C2)C2=CC=CC=C2.[OH-].[NH4+]>>N1(C=NC2=C1C=CC=C2)C=2SC(=C(N2)C2=CC=CC=C2)C(=O)N
CCO[C:2](=[O:3])[c:4]1[s:5][c:6](-[n:7]2[cH:8][n:9][c:10]3[cH:11][cH:12][cH:13][cH:14][c:15]23)[n:16][c:17]1-[c:18]1[cH:19][cH:20][cH:21][cH:22][cH:23]1.[NH4+:1]>>[NH2:1][C:2](=[O:3])[c:4]1[s:5][c:6](-[n:7]2[cH:8][n:9][c:10]3[cH:11][cH:12][cH:13][cH:14][c:15]23)[n:16][c:17]1-[c:18]1[cH:19][cH:20][cH:21][cH:22][cH:23]1
CCOC(=O)c1sc(-n2cnc3ccccc32)nc1-c1ccccc1.[NH4+]
NC(=O)c1sc(-n2cnc3ccccc32)nc1-c1ccccc1
null
null
null
Acylation
OtherReaction
d5b10d4f469e7a196a3b04a6a9e159a7d90514b6df5b50c1197d4b1b774c04e1
adc0ef6f6c1340dd2dbab737c85bf17fc842769181c5db1a2b4f82b391b28f9f
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8].[NH4+;D0:9]>>[NH2;D1;+0:9]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8]
13
[{"value": 13.0, "product": "N1(C=NC2=C1C=CC=C2)C=2SC(=C(N2)C2=CC=CC=C2)C(=O)N", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
2-Benzoimidazol-1-yl-4-phenyl-thiazole-5-carboxylic acid amide was prepared from 2-Benzoimidazol-1-yl-4-phenyl-thiazole-5-carboxylic acid ethyl ester (75 mg, 0.21 mmol) and ammonium hydroxide as described above in the general amide formation procedure. Preparative HPLC with trifluoroacetic acid, 9.1 mg, 13% yield. MS M...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary amide
null
null
c1cscn1.c1ccc2[nH]cnc2c1.c1ccccc1
HO-
null
null
null
CCOC(=O)c1sc(-n2cnc3ccccc32)nc1-c1ccccc1.[NH4+]>>NC(=O)c1sc(-n2cnc3ccccc32)nc1-c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f6a29c8c6eea4dfdba4d9337dde91421
CCOC(=O)c1sc(Cl)nc1-c1ccccc1.Cc1cc2nc[nH]c2cc1C>>Cc1cc2ncn(-c3nc(-c4ccccc4)c(C(=O)O)s3)c2cc1C
CC1=CC2=C(N=CN2)C=C1C.C(C)OC(=O)C1=C(N=C(S1)Cl)C1=CC=CC=C1>>CC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=CC=C2)C(=O)O)C=C1C
CC[O:20][C:18]([c:17]1[c:10](-[c:11]2[cH:12][cH:13][cH:14][cH:15][cH:16]2)[n:9][c:8](Cl)[s:21]1)=[O:19].[CH3:1][c:2]1[cH:3][c:4]2[n:5][cH:6][nH:7][c:22]2[cH:23][c:24]1[CH3:25]>>[CH3:1][c:2]1[cH:3][c:4]2[n:5][cH:6][n:7](-[c:8]3[n:9][c:10](-[c:11]4[cH:12][cH:13][cH:14][cH:15][cH:16]4)[c:17]([C:18](=[O:19])[OH:20])[s:21]3...
CCOC(=O)c1sc(Cl)nc1-c1ccccc1.Cc1cc2nc[nH]c2cc1C
Cc1cc2ncn(-c3nc(-c4ccccc4)c(C(=O)O)s3)c2cc1C
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
ec8532a11ed9b83fbbba3bdf52733b203d59017a181516e3b19fc619199ea16f
73d3046582ebe4ceb7e2b5dab4179dafc796946799b04fa5a989e4e71d346a3b
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]1:[#16;a:5]:[c;H0;D3;+0:6](-Cl):[#7;a:7]:[c:8]:1.[c:9]:[c:10]1:[nH;D2;+0:11]:[c:12]:[#7;a:13]:[c:14]:1:[c:15]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]1:[#16;a:5]:[c;H0;D3;+0:6](-[n;H0;D3;+0:11]2:[c:12]:[#7;a:13]:[c:14](:[c:15]):[c:10]:2:[c:9]):[#7;a:7]:[c:8]:1
null
[]
null
null
null
null
2-(5,6-Dimethylbenzoimidazol-1-yl)-4-phenylthiazole-5-carboxylic acid was prepared in a similar manner as that for Example 1 starting with the reaction of 5,6-dimethylbenzoimidazole and 2-Chloro-4-phenylthiazole-5-carboxylic acid ethyl ester. 1H-NMR(DMSO-D6) 8.82 (s, 1H); 7.98 (s, 1H); 7.82-7.92 (m, 2H); 7.58 (s, 1H); ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester
Carboxylic acid
c1cscn1.c1ccc2[nH]cnc2c1
c1ccc2[nH]cnc2c1.c1cscn1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1
HCl
null
null
null
CCOC(=O)c1sc(Cl)nc1-c1ccccc1.Cc1cc2nc[nH]c2cc1C>>Cc1cc2ncn(-c3nc(-c4ccccc4)c(C(=O)O)s3)c2cc1C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-32c6f14ec2074983be4c1949f91105d3
CCOC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1.N>>COc1cc2ncn(-c3nc(-c4ccccc4)c(C(N)=O)s3)c2cc1OC
C(C)OC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC=CC=C2.N>>COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=CC=C2)C(=O)N)C=C1OC
CCO[C:19]([c:18]1[c:11](-[c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:25]([O:26][CH3:27])[cH:24][c:23]32)[s:22]1)=[O:21].[NH3:20]>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][cH:15][cH:16][cH:17]4)[c:18]([C:19](...
CCOC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1.N
COc1cc2ncn(-c3nc(-c4ccccc4)c(C(N)=O)s3)c2cc1OC
null
null
C(C)O
Acylation
OtherReaction
d5b10d4f469e7a196a3b04a6a9e159a7d90514b6df5b50c1197d4b1b774c04e1
adc0ef6f6c1340dd2dbab737c85bf17fc842769181c5db1a2b4f82b391b28f9f
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8].[NH3;D0;+0:9]>>[NH2;D1;+0:9]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8]
36
[{"value": 36.0, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=CC=C2)C(=O)N)C=C1OC", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-phenyl-thiazole-5-carboxylic acid amide was prepared from 2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-phenyl-thiazole-5-carboxylic acid ethyl ester (80 mg, 0.20 mmol) and ammonia in ethanol (29 molar) as described above in the general amide formation procedure. The product was isolated...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary amide
null
null
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1
HO-
C(C)O
null
null
CCOC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1.N>C(C)O>COc1cc2ncn(-c3nc(-c4ccccc4)c(C(N)=O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-613b1935d1d64b12be7ea78814253fd8
CCOC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1.CNC>>COc1cc2ncn(-c3nc(-c4ccccc4)c(C(=O)N(C)C)s3)c2cc1OC
C(C)OC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC=CC=C2.CNC>>CN(C(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC=CC=C2)C
CCO[C:19]([c:18]1[c:11](-[c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:27]([O:28][CH3:29])[cH:26][c:25]32)[s:24]1)=[O:20].[NH:21]([CH3:22])[CH3:23]>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][cH:15][cH:16][cH:17...
CCOC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1.CNC
COc1cc2ncn(-c3nc(-c4ccccc4)c(C(=O)N(C)C)s3)c2cc1OC
null
null
CO
Acylation
Aminolysis of esters
d147787750807073759132276086de98566af6772417f9288b6300bf1de7801c
fa66342dd118fe5531ba6a998ac8fab92d2b0db4fd04688560eec7d04e9be0e4
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8].[C;D1;H3:9]-[NH;D2;+0:10]-[C;D1;H3:11]>>[C;D1;H3:9]-[N;H0;D3;+0:10](-[C;D1;H3:11])-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8]
null
[]
null
null
null
null
2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-phenyl-thiazole-5-carboxylic acid dimethylamide was prepared from 2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-phenyl-thiazole-5-carboxylic acid ethyl ester (48.8 mg, 0.12 mmol) and dimethyl amine in methanol (2 molar) as described above in the general amide formation procedure. Product...
10.6084/m9.figshare.5104873.v1
null
Ester.Secondary amine
Tertiary amide
null
null
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1
HO-
CO
null
null
CCOC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1.CNC>CO>COc1cc2ncn(-c3nc(-c4ccccc4)c(C(=O)N(C)C)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-bab919471b49460297e5e432b8cbb56a
CCN.CCOC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1>>CCNC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1
C(C)OC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC=CC=C2.C(C)N>>C(C)NC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC=CC=C2
[CH3:1][CH2:2][NH2:3].CCO[C:4](=[O:5])[c:6]1[s:7][c:8](-[n:9]2[cH:10][n:11][c:12]3[cH:13][c:14]([O:15][CH3:16])[c:17]([O:18][CH3:19])[cH:20][c:21]23)[n:22][c:23]1-[c:24]1[cH:25][cH:26][cH:27][cH:28][cH:29]1>>[CH3:1][CH2:2][NH:3][C:4](=[O:5])[c:6]1[s:7][c:8](-[n:9]2[cH:10][n:11][c:12]3[cH:13][c:14]([O:15][CH3:16])[c:17]...
CCN.CCOC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1
CCNC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1
null
null
CO
Acylation
Aminolysis of esters
04c54ce22aa9bc0cea0de3d900446bcab51cf02bebeb606fa788a47dcd0e37ff
4335147c9ad02004b7c12428d7eac0b2e7e0e2017adc471d01c387239de8017d
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8].[C;D1;H3:9]-[C:10]-[NH2;D1;+0:11]>>[C;D1;H3:9]-[C:10]-[NH;D2;+0:11]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8]
null
[]
null
null
null
null
2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-phenyl-thiazole-5-carboxylic acid ethylamide was prepared from 2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-phenyl-thiazole-5-carboxylic acid ethyl ester (30 mg, 0.07 mmol) and ethylamine in methanol (2 molar) as described above in the general amide formation procedure. Product was isol...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine
Secondary amide
null
null
c1cscn1.c1ccc2[nH]cnc2c1.c1ccccc1
HO-
CO
null
null
CCN.CCOC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1>CO>CCNC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d612e4db810f4c038452da2bbc6fc150
CCOC(=O)c1sc(Cl)nc1-c1ccccc1>>O=C(O)c1sc(Cl)nc1-c1ccccc1
C(C)OC(=O)C1=C(N=C(S1)Cl)C1=CC=CC=C1>>ClC=1SC(=C(N1)C1=CC=CC=C1)C(=O)O
CC[O:3][C:2](=[O:1])[c:4]1[s:5][c:6]([Cl:7])[n:8][c:9]1-[c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1>>[O:1]=[C:2]([OH:3])[c:4]1[s:5][c:6]([Cl:7])[n:8][c:9]1-[c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1
CCOC(=O)c1sc(Cl)nc1-c1ccccc1
O=C(O)c1sc(Cl)nc1-c1ccccc1
null
null
O1CCCC1.[OH-].[Na+]
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(-c2cscn2)cc1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4](:[#16;a:5]):[c:6]:[#7;a:7]>>[#16;a:5]:[c:4](-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]):[c:6]:[#7;a:7]
92.6
[{"value": 35.0, "product": "ClC=1SC(=C(N1)C1=CC=CC=C1)C(=O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 92.6, "product": "ClC=1SC(=C(N1)C1=CC=CC=C1)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
A mixture of 2-Chloro-4-phenyl-thiazole-5-carboxylic acid ethyl ester (1 g, 3.74 mmol) in tetrahydrofuran (10 ml) and NaOH (15%, 4.8 ml) was stirred at room temperature for 2 hr. After removal of tetrahydrofuran, the aqueous was neutralized with aqueous hydrochloric acid (3 N) to ˜pH=3. The solid was filtered and washe...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1cscn1.c1ccccc1
Other
O1CCCC1.[OH-].[Na+]
null
2
CCOC(=O)c1sc(Cl)nc1-c1ccccc1>O1CCCC1.[OH-].[Na+]>O=C(O)c1sc(Cl)nc1-c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-99f1d4865b4b4902a6aeeb9077daab74
COc1cc2nc[nH]c2cc1OC.N#Cc1sc(Cl)nc1-c1ccccc1>>COc1cc2ncn(-c3nc(-c4ccccc4)c(C#N)s3)c2cc1OC
COC1=CC2=C(N=CN2)C=C1OC.ClC=1SC(=C(N1)C1=CC=CC=C1)C#N.N1C=NC=2C1=CC=1COCOC1C2>>COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=CC=C2)C#N)C=C1OC
[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][nH:8][c:22]2[cH:23][c:24]1[O:25][CH3:26].Cl[c:9]1[n:10][c:11](-[c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[c:18]([C:19]#[N:20])[s:21]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][cH:15][cH:16][cH:17]4)[c:18]([C:19]#[N:20])[s:21]3)...
COc1cc2nc[nH]c2cc1OC.N#Cc1sc(Cl)nc1-c1ccccc1
COc1cc2ncn(-c3nc(-c4ccccc4)c(C#N)s3)c2cc1OC
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
b38f76237cdec2baf41c9411839797fed979828e4dd9354fb2aa8a56efaef6ba
e3660767655c50df0f92afc78c794dd2af7cf646bf1430960eafd30c23bf3fa7
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Cl-[c;H0;D3;+0:1]1:[#16;a:2]:[c:3]:[c:4]:[#7;a:5]:1.[c:6]:[c:7]1:[nH;D2;+0:8]:[c:9]:[#7;a:10]:[c:11]:1:[c:12]>>[c:6]:[c:7]1:[c:11](:[c:12]):[#7;a:10]:[c:9]:[n;H0;D3;+0:8]:1-[c;H0;D3;+0:1]1:[#16;a:2]:[c:3]:[c:4]:[#7;a:5]:1
47
[{"value": 47.0, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=CC=C2)C#N)C=C1OC", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-phenyl-thiazole-5-carbonitrile (48.8 mg, yield 47%) was prepared from 5,6-dimethoxybenzimidazole (76 mg, 0.43 mmol) and 2-chloro-4-phenyl-thiazole-5-carbonitrile as described in Example 1 (63 mg, 0.28 mmol). MS M/z 363 (M+1) Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1ccc2[nH]cnc2c1.c1cscn1
c1ccc2[nH]cnc2c1.c1cscn1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1
HCl
null
null
null
COc1cc2nc[nH]c2cc1OC.N#Cc1sc(Cl)nc1-c1ccccc1>>COc1cc2ncn(-c3nc(-c4ccccc4)c(C#N)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-fb6e880335694781a11645def0a210f7
COc1cc2ncn(-c3nc(-c4ccccc4)c(C#N)s3)c2cc1OC.[N-]=[N+]=[N-]>>COc1cc2ncn(-c3nc(-c4ccccc4)c(-c4nnn[nH]4)s3)c2cc1OC
O.COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=CC=C2)C#N)C=C1OC.[N-]=[N+]=[N-].[Na+].[Cl-].[NH4+]>>COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=CC=C2)C2=NN=NN2)C=C1OC
[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][cH:15][cH:16][cH:17]4)[c:18]([C:19]#[N:20])[s:24]3)[c:25]2[cH:26][c:27]1[O:28][CH3:29].[N-:21]=[N+:22]=[N-:23]>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][cH:15][cH:16][cH:17]4)[c:18]...
COc1cc2ncn(-c3nc(-c4ccccc4)c(C#N)s3)c2cc1OC.[N-]=[N+]=[N-]
COc1cc2ncn(-c3nc(-c4ccccc4)c(-c4nnn[nH]4)s3)c2cc1OC
null
null
CN1C(CCC1)=O
Aromatic Heterocycle Formation
OtherReaction
237b84aaa459abf427f233dc6a07a1d9de824f980714e458423189bb68f60f12
d8c808528b7ee68720aaeebd35cb6a2a30e344748d0066102cdae99843b93cf0
c1ccc(-c2nc(-n3cnc4ccccc43)sc2-c2nnn[nH]2)cc1
[#7;a:1]:[c:2]:[#7;a:3]-[c:4]1:[#16;a:5]:[c;H0;D3;+0:6](-[C;H0;D2;+0:7]#[N;H0;D1;+0:8]):[c:9](-[c:10]):[#7;a:11]:1.[N-;H0;D1:12]=[N+;H0;D2:13]=[N-;H0;D1:14]>>[#7;a:1]:[c:2]:[#7;a:3]-[c:4]1:[#16;a:5]:[c;H0;D3;+0:6](-[c;H0;D3;+0:7]2:[n;H0;D2;+0:8]:[n;H0;D2;+0:12]:[n;H0;D2;+0:13]:[nH;D2;+0:14]:2):[c:9](-[c:10]):[#7;a:11]:...
47.3
[{"value": 47.0, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=CC=C2)C2=NN=NN2)C=C1OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 47.3, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=CC=C2)C2=NN=NN2)C=C1OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
110
CELSIUS
1
HOUR
A mixture of 2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-phenyl-thiazole-5-carbonitrile (261 mg, 0.72 mmol), sodium azide (220 mg) and ammonium chloride (250 mg) in N-methylpyrrolidone (2.5 ml) was stirred at 110° C. for 1 hr. Water was added and the mixture was extracted with methylene chloride. After removal of solvent, t...
10.6084/m9.figshare.5104873.v1
null
Nitrile
null
null
c1nnn[nH]1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1.c1nnn[nH]1
null
CN1C(CCC1)=O
110
1
COc1cc2ncn(-c3nc(-c4ccccc4)c(C#N)s3)c2cc1OC.[N-]=[N+]=[N-]>CN1C(CCC1)=O>COc1cc2ncn(-c3nc(-c4ccccc4)c(-c4nnn[nH]4)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ce90a2564f46480babd0cc3e1ace11c7
CCOC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1.NC1CC1>>COc1cc2ncn(-c3nc(-c4ccccc4)c(C(=O)NC4CC4)s3)c2cc1OC
C(C)OC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC=CC=C2.C1(CC1)N>>C1(CC1)NC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC=CC=C2
CCO[C:19]([c:18]1[c:11](-[c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:28]([O:29][CH3:30])[cH:27][c:26]32)[s:25]1)=[O:20].[NH2:21][CH:22]1[CH2:23][CH2:24]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][cH:15][cH:1...
CCOC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1.NC1CC1
COc1cc2ncn(-c3nc(-c4ccccc4)c(C(=O)NC4CC4)s3)c2cc1OC
null
null
CO
Acylation
Aminolysis of esters
04c54ce22aa9bc0cea0de3d900446bcab51cf02bebeb606fa788a47dcd0e37ff
4335147c9ad02004b7c12428d7eac0b2e7e0e2017adc471d01c387239de8017d
O=C(NC1CC1)c1sc(-n2cnc3ccccc32)nc1-c1ccccc1
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8].[NH2;D1;+0:9]-[C:10]1-[C:11]-[C:12]-1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:9]-[C:10]1-[C:11]-[C:12]-1)-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8]
null
[]
null
null
null
null
2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-phenyl-thiazole-5-carboxylic acid cyclopropylamide was prepared from 2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-phenyl-thiazole-5-carboxylic acid ethyl ester (24 mg, 0.06 mmol) and cyclopropylamine in methanol (4 molar) as described above in the general amide formation procedure. Prod...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine
Secondary amide
null
null
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1.C1CC1
HO-
CO
null
null
CCOC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1.NC1CC1>CO>COc1cc2ncn(-c3nc(-c4ccccc4)c(C(=O)NC4CC4)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-950ff29ccb2f4da8b36cb7e8427e747f
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.COc1ccc(B(O)O)cc1OC>>COc1ccc(-c2nc(-n3cnc4cc(OC)c(OC)cc43)sc2C(=O)O)cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.COC=1C=C(C=CC1OC)B(O)O>>COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=C(C=C2)OC)OC)C(=O)O)C=C1OC
C[O:27][C:25]([c:24]1[c:7](Br)[n:8][c:9](-[n:10]2[cH:11][n:12][c:13]3[cH:14][c:15]([O:16][CH3:17])[c:18]([O:19][CH3:20])[cH:21][c:22]23)[s:23]1)=[O:26].OB(O)[c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[c:29]([O:30][CH3:31])[cH:28]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[n:8][c:9](-[n:10]3[cH:11][n:12][c:13]4[cH:14][c:15...
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.COc1ccc(B(O)O)cc1OC
COc1ccc(-c2nc(-n3cnc4cc(OC)c(OC)cc43)sc2C(=O)O)cc1OC
null
null
null
C-C Coupling
OtherReaction
f263884194c3689072b842d9444db2ca155af322288a9afe28e6da9e83653e3c
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]>>[O;D1;H0:7]=[C:6](-[OH;D1;+0:8])-[c:5]1:[#16;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]
60
[{"value": 60.0, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=C(C=C2)OC)OC)C(=O)O)C=C1OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 59.8, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=C(C=C2)OC)OC)C(=O)O)C=C1OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and 3,4-dimethoxyphenylboronic acid (27.3 mg, 0.15 mmol) gave 2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-(3,4-dimethoxy-phenyl)-thiazole-5-carboxylic acid (26.4 mg, 60%) as...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1cscn1.c1ccccc1
c1ccccc1.c1cscn1
c1ccccc1.c1cscn1.c1ccc2[nH]cnc2c1
HBr.B
null
null
null
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.COc1ccc(B(O)O)cc1OC>>COc1ccc(-c2nc(-n3cnc4cc(OC)c(OC)cc43)sc2C(=O)O)cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a43f73ea71054f398ab5c17438a8a78b
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccc(F)c(Cl)c1>>COc1cc2ncn(-c3nc(-c4ccc(F)c(Cl)c4)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.ClC=1C=C(C=CC1F)B(O)O>>ClC=1C=C(C=CC1F)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC
C[O:23][C:21]([c:20]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:27]([O:28][CH3:29])[cH:26][c:25]32)[s:24]1)=[O:22].OB(O)[c:12]1[cH:13][cH:14][c:15]([F:16])[c:17]([Cl:18])[cH:19]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][c:15]([F:16])[c:17]...
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccc(F)c(Cl)c1
COc1cc2ncn(-c3nc(-c4ccc(F)c(Cl)c4)c(C(=O)O)s3)c2cc1OC
null
null
null
C-C Coupling
OtherReaction
f263884194c3689072b842d9444db2ca155af322288a9afe28e6da9e83653e3c
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]>>[O;D1;H0:7]=[C:6](-[OH;D1;+0:8])-[c:5]1:[#16;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]
19
[{"value": 19.0, "product": "ClC=1C=C(C=CC1F)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 18.9, "product": "ClC=1C=C(C=CC1F)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and 3-chloro-4-fluorophenylboronic acid (26.2 mg, 0.15 mmol) gave 4-(3-Chloro-4-fluoro-phenyl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid (8.2 mg, ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1cscn1.c1ccccc1
c1cscn1.c1ccccc1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1
HBr.B
null
null
null
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccc(F)c(Cl)c1>>COc1cc2ncn(-c3nc(-c4ccc(F)c(Cl)c4)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-879b0c927d714358b78bab6d425e821d
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccc(F)c1>>COc1cc2ncn(-c3nc(-c4cccc(F)c4)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.FC=1C=C(C=CC1)B(O)O>>COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=CC=C2)F)C(=O)O)C=C1OC
C[O:22][C:20]([c:19]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:26]([O:27][CH3:28])[cH:25][c:24]32)[s:23]1)=[O:21].OB(O)[c:12]1[cH:13][cH:14][cH:15][c:16]([F:17])[cH:18]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][cH:15][c:16]([F:17])[cH:18]...
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccc(F)c1
COc1cc2ncn(-c3nc(-c4cccc(F)c4)c(C(=O)O)s3)c2cc1OC
null
null
null
C-C Coupling
OtherReaction
f263884194c3689072b842d9444db2ca155af322288a9afe28e6da9e83653e3c
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]>>[O;D1;H0:7]=[C:6](-[OH;D1;+0:8])-[c:5]1:[#16;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]
20
[{"value": 20.0, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=CC=C2)F)C(=O)O)C=C1OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 19.5, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=CC=C2)F)C(=O)O)C=C1OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and 3-fluorophenylboronic acid (21 mg, 0.15 mmol) gave 2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-(3-fluoro-phenyl)-thiazole-5-carboxylic acid (7.8 mg, 20%) as a white soli...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1cscn1.c1ccccc1
c1cscn1.c1ccccc1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1
HBr.B
null
null
null
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccc(F)c1>>COc1cc2ncn(-c3nc(-c4cccc(F)c4)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0c432ad6e03a4d1ea75e44ac91761844
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccccc1Cl>>COc1cc2ncn(-c3nc(-c4ccccc4Cl)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.ClC1=C(C=CC=C1)B(O)O>>ClC1=C(C=CC=C1)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC
C[O:22][C:20]([c:19]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:26]([O:27][CH3:28])[cH:25][c:24]32)[s:23]1)=[O:21].OB(O)[c:12]1[cH:13][cH:14][cH:15][cH:16][c:17]1[Cl:18]>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][cH:15][cH:16][c:17]4[Cl:18])...
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccccc1Cl
COc1cc2ncn(-c3nc(-c4ccccc4Cl)c(C(=O)O)s3)c2cc1OC
null
null
null
C-C Coupling
OtherReaction
f263884194c3689072b842d9444db2ca155af322288a9afe28e6da9e83653e3c
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12](-[Cl;D1;H0:13]):[c:14]>>[Cl;D1;H0:13]-[c:12](:[c:14]):[c;H0;D3;+0:9](-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[OH;D1;+0:8]):[c:10]:[c:11]
46.2
[{"value": 46.0, "product": "ClC1=C(C=CC=C1)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 46.2, "product": "ClC1=C(C=CC=C1)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and 2-chlorophenylboronic acid (23.5 mg, 0.15 mmol) gave 4-(2-Chloro-phenyl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid (19.2 mg, 46%) as a white s...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1cscn1.c1ccccc1
c1cscn1.c1ccccc1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1
HBr.B
null
null
null
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccccc1Cl>>COc1cc2ncn(-c3nc(-c4ccccc4Cl)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1ab497d711da436ea193882c249cc4ab
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccc2c(c1)OCO2>>COc1cc2ncn(-c3nc(-c4ccc5c(c4)OCO5)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.C1OC=2C=C(C=CC2O1)B(O)O>>O1COC2=C1C=CC(=C2)C=2N=C(SC2C(=O)O)N2C=NC1=C2C=C(C(=C1)OC)OC
C[O:24][C:22]([c:21]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:28]([O:29][CH3:30])[cH:27][c:26]32)[s:25]1)=[O:23].OB(O)[c:12]1[cH:13][cH:14][c:15]2[c:16]([cH:17]1)[O:18][CH2:19][O:20]2>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][c:15]5[c:16]...
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccc2c(c1)OCO2
COc1cc2ncn(-c3nc(-c4ccc5c(c4)OCO5)c(C(=O)O)s3)c2cc1OC
null
null
null
C-C Coupling
OtherReaction
2be91abefca374375f70d11b43d2684970780fd1d29fcf5da44605ad13137d6c
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc2c(c1)ncn2-c1nc(-c2ccc3c(c2)OCO3)cs1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]-[#8:14]>>[#8:14]-[c:13]:[c:12]:[c;H0;D3;+0:9](-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[OH;D1;+0:8]):[c:10]:[c:11]
25
[{"value": 25.0, "product": "O1COC2=C1C=CC(=C2)C=2N=C(SC2C(=O)O)N2C=NC1=C2C=C(C(=C1)OC)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 24.7, "product": "O1COC2=C1C=CC(=C2)C=2N=C(SC2C(=O)O)N2C=NC1=C2C=C(C(=C1)OC)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and 3,4-methylenedioxybenzeneboronic acid (24.9 mg, 0.15 mmol) gave 4-Benzo[1,3]dioxol-5-yl-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid (10.5 mg, 25...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1cscn1.c1ccc2c(c1)OCO2
c1cscn1.c1ccc2c(c1)OCO2
c1ccc2[nH]cnc2c1.c1cscn1.c1ccc2c(c1)OCO2
HBr.B
null
null
null
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccc2c(c1)OCO2>>COc1cc2ncn(-c3nc(-c4ccc5c(c4)OCO5)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e714197cb214499fa47edb8ecbbac83d
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccc(Cl)c(Cl)c1>>COc1cc2ncn(-c3nc(-c4ccc(Cl)c(Cl)c4)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.ClC=1C=C(C=CC1Cl)B(O)O>>ClC=1C=C(C=CC1Cl)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC
C[O:23][C:21]([c:20]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:27]([O:28][CH3:29])[cH:26][c:25]32)[s:24]1)=[O:22].OB(O)[c:12]1[cH:13][cH:14][c:15]([Cl:16])[c:17]([Cl:18])[cH:19]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][c:15]([Cl:16])[c:1...
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccc(Cl)c(Cl)c1
COc1cc2ncn(-c3nc(-c4ccc(Cl)c(Cl)c4)c(C(=O)O)s3)c2cc1OC
null
null
null
C-C Coupling
OtherReaction
f263884194c3689072b842d9444db2ca155af322288a9afe28e6da9e83653e3c
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]>>[O;D1;H0:7]=[C:6](-[OH;D1;+0:8])-[c:5]1:[#16;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]
35.3
[{"value": 35.0, "product": "ClC=1C=C(C=CC1Cl)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 35.3, "product": "ClC=1C=C(C=CC1Cl)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and 3,4-dichlorophenylboronic acid (28.6 mg, 0.15 mmol) gave 4-(3,4-Dichloro-phenyl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid (15.9 mg, 35%) as a...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1cscn1.c1ccccc1
c1cscn1.c1ccccc1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1
HBr.B
null
null
null
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccc(Cl)c(Cl)c1>>COc1cc2ncn(-c3nc(-c4ccc(Cl)c(Cl)c4)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3a8fbc60df854bfdaf019653858ba679
CC(C)c1cccc(B(O)O)c1.COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br>>COc1cc2ncn(-c3nc(-c4cccc(C(C)C)c4)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.C(C)(C)C=1C=C(C=CC1)B(O)O>>COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=CC=C2)C(C)C)C(=O)O)C=C1OC
OB(O)[c:12]1[cH:13][cH:14][cH:15][c:16]([CH:17]([CH3:18])[CH3:19])[cH:20]1.C[O:24][C:22]([c:21]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:28]([O:29][CH3:30])[cH:27][c:26]32)[s:25]1)=[O:23]>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][cH:15][c...
CC(C)c1cccc(B(O)O)c1.COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br
COc1cc2ncn(-c3nc(-c4cccc(C(C)C)c4)c(C(=O)O)s3)c2cc1OC
null
null
null
C-C Coupling
OtherReaction
f263884194c3689072b842d9444db2ca155af322288a9afe28e6da9e83653e3c
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]>>[O;D1;H0:7]=[C:6](-[OH;D1;+0:8])-[c:5]1:[#16;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]
44
[{"value": 44.0, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=CC=C2)C(C)C)C(=O)O)C=C1OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 43.9, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=CC=C2)C(C)C)C(=O)O)C=C1OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and 3-isopropylphenylboronic acid (24.6 mg, 0.15 mmol) gave 2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-(3-isopropyl-phenyl)-thiazole-5-carboxylic acid (18.6 mg, 44%) as a w...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1ccccc1.c1cscn1
c1cscn1.c1ccccc1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1
HBr.B
null
null
null
CC(C)c1cccc(B(O)O)c1.COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br>>COc1cc2ncn(-c3nc(-c4cccc(C(C)C)c4)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-202afac41ead4155b0e6e8530a84c2c9
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccsc1>>COc1cc2ncn(-c3nc(-c4ccsc4)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.S1C=C(C=C1)B(O)O>>COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CSC=C2)C(=O)O)C=C1OC
C[O:20][C:18]([c:17]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:24]([O:25][CH3:26])[cH:23][c:22]32)[s:21]1)=[O:19].OB(O)[c:12]1[cH:13][cH:14][s:15][cH:16]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][s:15][cH:16]4)[c:17]([C:18](=[O:19])[OH:20...
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccsc1
COc1cc2ncn(-c3nc(-c4ccsc4)c(C(=O)O)s3)c2cc1OC
null
null
null
C-C Coupling
OtherReaction
0ed2d1457ada7a09f0b8cc1706b21f6fab34ba9c2452322a30b35a2c41d1fe63
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc2c(c1)ncn2-c1nc(-c2ccsc2)cs1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9]1:[c:10]:[c:11]:[#16;a:12]:[c:13]:1>>[O;D1;H0:7]=[C:6](-[OH;D1;+0:8])-[c:5]1:[#16;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:9]1:[c:10]:[c:11]:[#16;a:12]:[c:13]:1
78
[{"value": 78.0, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CSC=C2)C(=O)O)C=C1OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 77.7, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CSC=C2)C(=O)O)C=C1OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and thiophene-3-boronic acid (19.2 mg, 0.15 mmol) gave 2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-thiophen-3-yl-thiazole-5-carboxylic acid (30.1 mg, 78%) as a white solid. ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1cscn1.c1ccsc1
c1cscn1.c1ccsc1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccsc1
HBr.B
null
null
null
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccsc1>>COc1cc2ncn(-c3nc(-c4ccsc4)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-97e1be71531e4514a0017251a3ba16db
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.Cc1ccc(B(O)O)cc1>>COc1cc2ncn(-c3nc(-c4ccc(C)cc4)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.CC1=CC=C(C=C1)B(O)O.C(=O)([O-])[O-].[Na+].[Na+].[OH-].[Na+]>>COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=C(C=C2)C)C(=O)O)C=C1OC
C[O:22][C:20]([c:19]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:26]([O:27][CH3:28])[cH:25][c:24]32)[s:23]1)=[O:21].OB(O)[c:12]1[cH:13][cH:14][c:15]([CH3:16])[cH:17][cH:18]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][c:15]([CH3:16])[cH:17][cH...
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.Cc1ccc(B(O)O)cc1
COc1cc2ncn(-c3nc(-c4ccc(C)cc4)c(C(=O)O)s3)c2cc1OC
null
C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.Cl[Pd]Cl.[Fe+2]
O.COCCOC.CO.C1CCOC1
C-C Coupling
OtherReaction
f263884194c3689072b842d9444db2ca155af322288a9afe28e6da9e83653e3c
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]>>[O;D1;H0:7]=[C:6](-[OH;D1;+0:8])-[c:5]1:[#16;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]
53.4
[{"value": 53.0, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=C(C=C2)C)C(=O)O)C=C1OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 53.4, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=C(C=C2)C)C(=O)O)C=C1OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
null
null
To a solution of 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol), 4-methylphenylboronic acid (20.4 mg, 0.15 mmol) in ethylene glycol dimethyl ether (1 ml) was added Na2CO3 (2M, 100 μL, 0.2 mmol) and [1,1′-bis(diphenylphosphino)-ferrocene]dichloro palladium(II) (4 m...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1cscn1.c1ccccc1
c1cscn1.c1ccccc1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1
HBr.B
C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.Cl[Pd]Cl.[Fe+2].O.COCCOC.CO.C1CCOC1
100
null
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.Cc1ccc(B(O)O)cc1>C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.Cl[Pd]Cl.[Fe+2].O.COCCOC.CO.C1CCOC1>COc1cc2ncn(-c3nc(-c4ccc(C)cc4)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-235ff213f38548958d27e1579ebdf497
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.Cc1ccccc1B(O)O>>COc1cc2ncn(-c3nc(-c4ccccc4C)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.CC1=C(C=CC=C1)B(O)O>>COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=C(C=CC=C2)C)C(=O)O)C=C1OC
C[O:22][C:20]([c:19]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:26]([O:27][CH3:28])[cH:25][c:24]32)[s:23]1)=[O:21].OB(O)[c:12]1[cH:13][cH:14][cH:15][cH:16][c:17]1[CH3:18]>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][cH:15][cH:16][c:17]4[CH3:18...
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.Cc1ccccc1B(O)O
COc1cc2ncn(-c3nc(-c4ccccc4C)c(C(=O)O)s3)c2cc1OC
null
null
null
C-C Coupling
OtherReaction
f263884194c3689072b842d9444db2ca155af322288a9afe28e6da9e83653e3c
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12](-[C;D1;H3:13]):[c:14]>>[C;D1;H3:13]-[c:12](:[c:14]):[c;H0;D3;+0:9](-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[OH;D1;+0:8]):[c:10]:[c:11]
57
[{"value": 57.0, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=C(C=CC=C2)C)C(=O)O)C=C1OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 56.9, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=C(C=CC=C2)C)C(=O)O)C=C1OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and 2-methylphenylboronic acid (20.4 mg, 0.15 mmol) gave 2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-o-tolyl-thiazole-5-carboxylic acid (22.5 mg, 57%) as a white solid. 1H N...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1cscn1.c1ccccc1
c1cscn1.c1ccccc1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1
HBr.B
null
null
null
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.Cc1ccccc1B(O)O>>COc1cc2ncn(-c3nc(-c4ccccc4C)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-bd991cebe8ea4376aafae9d62ce28f18
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccc(F)c1F>>COc1cc2ncn(-c3nc(-c4cccc(F)c4F)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.FC1=C(C=CC=C1F)B(O)O>>FC1=C(C=CC=C1F)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC
C[O:23][C:21]([c:20]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:27]([O:28][CH3:29])[cH:26][c:25]32)[s:24]1)=[O:22].OB(O)[c:12]1[cH:13][cH:14][cH:15][c:16]([F:17])[c:18]1[F:19]>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][cH:15][c:16]([F:17])[c...
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccc(F)c1F
COc1cc2ncn(-c3nc(-c4cccc(F)c4F)c(C(=O)O)s3)c2cc1OC
null
null
null
C-C Coupling
OtherReaction
f263884194c3689072b842d9444db2ca155af322288a9afe28e6da9e83653e3c
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12](-[F;D1;H0:13]):[c:14]>>[F;D1;H0:13]-[c:12](:[c:14]):[c;H0;D3;+0:9](-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[OH;D1;+0:8]):[c:10]:[c:11]
39
[{"value": 39.0, "product": "FC1=C(C=CC=C1F)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and 2,3-difluorophenylboronic acid (23.7 mg, 0.15 mmol) gave 4-(2,3-Difluoro-phenyl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid (16.2 39%) as a whi...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1cscn1.c1ccccc1
c1cscn1.c1ccccc1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1
HBr.B
null
null
null
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccc(F)c1F>>COc1cc2ncn(-c3nc(-c4cccc(F)c4F)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d9360d4309a44ed58a73f5b3e79e0c3c
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccc(Cl)c1>>COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.ClC=1C=C(C=CC1)B(O)O>>ClC=1C=C(C=CC1)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC
C[O:22][C:20]([c:19]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:26]([O:27][CH3:28])[cH:25][c:24]32)[s:23]1)=[O:21].OB(O)[c:12]1[cH:13][cH:14][cH:15][c:16]([Cl:17])[cH:18]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][cH:15][c:16]([Cl:17])[cH:1...
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccc(Cl)c1
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC
null
null
null
C-C Coupling
OtherReaction
f263884194c3689072b842d9444db2ca155af322288a9afe28e6da9e83653e3c
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]>>[O;D1;H0:7]=[C:6](-[OH;D1;+0:8])-[c:5]1:[#16;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]
21
[{"value": 21.0, "product": "ClC=1C=C(C=CC1)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 20.7, "product": "ClC=1C=C(C=CC1)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and 3-chlorophenylboronic acid (23.5 mg, 0.15 mmol) gave 4-(3-Chloro-phenyl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid (8.6 mg, 21%) as a white so...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1cscn1.c1ccccc1
c1cscn1.c1ccccc1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1
HBr.B
null
null
null
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccc(Cl)c1>>COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3443172873194b13957611ed3d24b997
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccc2ccccc12>>COc1cc2ncn(-c3nc(-c4cccc5ccccc45)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.C1(=CC=CC2=CC=CC=C12)B(O)O>>COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=CC3=CC=CC=C23)C(=O)O)C=C1OC
C[O:25][C:23]([c:22]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:29]([O:30][CH3:31])[cH:28][c:27]32)[s:26]1)=[O:24].OB(O)[c:12]1[cH:13][cH:14][cH:15][c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]12>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][cH:15]...
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccc2ccccc12
COc1cc2ncn(-c3nc(-c4cccc5ccccc45)c(C(=O)O)s3)c2cc1OC
null
null
null
C-C Coupling
OtherReaction
c249834ead4e53af5cb050a81f13edb2a5778f7b441ec14f26aa07d5710a04ba
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc2c(-c3csc(-n4cnc5ccccc54)n3)cccc2c1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12](:[c:13]):[c:14]>>[O;D1;H0:7]=[C:6](-[OH;D1;+0:8])-[c:5]1:[#16;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12](:[c:13]):[c:14]
37
[{"value": 37.0, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=CC3=CC=CC=C23)C(=O)O)C=C1OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 36.9, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=CC3=CC=CC=C23)C(=O)O)C=C1OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and 1-naphthaleneboronic acid (25.8 mg, 0.15 mmol) gave 2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-naphthalen-1-yl-thiazole-5-carboxylic acid (15.9 mg, 37%) as a white soli...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1cscn1.c1ccc2ccccc2c1
c1cscn1.c1ccc2ccccc2c1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccc2ccccc2c1
HBr.B
null
null
null
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccc2ccccc12>>COc1cc2ncn(-c3nc(-c4cccc5ccccc45)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9bbef3dc2cee4b7ea9e5066d534c6f9a
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccnc1>>COc1cc2ncn(-c3nc(-c4cccnc4)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.N1=CC(=CC=C1)B(O)O>>COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C=2C=NC=CC2)C(=O)O)C=C1OC
C[O:21][C:19]([c:18]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:25]([O:26][CH3:27])[cH:24][c:23]32)[s:22]1)=[O:20].OB(O)[c:12]1[cH:13][cH:14][cH:15][n:16][cH:17]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][cH:15][n:16][cH:17]4)[c:18]([C:19](...
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccnc1
COc1cc2ncn(-c3nc(-c4cccnc4)c(C(=O)O)s3)c2cc1OC
null
null
null
C-C Coupling
OtherReaction
58a128499e1cf40b3d2acb49265b500ef6547a0f5f09ed85c82cab43505a2ce6
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1cncc(-c2csc(-n3cnc4ccccc43)n2)c1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9]1:[c:10]:[c:11]:[c:12]:[#7;a:13]:[c:14]:1>>[O;D1;H0:7]=[C:6](-[OH;D1;+0:8])-[c:5]1:[#16;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:9]1:[c:10]:[c:11]:[c:12]:[#7;a:13]:[c:14]:1
7
[{"value": 7.0, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C=2C=NC=CC2)C(=O)O)C=C1OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 6.8, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C=2C=NC=CC2)C(=O)O)C=C1OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and pyridine-3-boronic acid (18.4 mg, 0.15 mmol) gave 2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-pyridin-3-yl-thiazole-5-carboxylic acid (2.6 mg, 7%) as a white solid. 1H N...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1cscn1.c1ccncc1
c1cscn1.c1ccncc1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccncc1
HBr.B
null
null
null
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccnc1>>COc1cc2ncn(-c3nc(-c4cccnc4)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5e3294a138ba401099617042607b4b46
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccc(O)c1>>COc1cc2ncn(-c3nc(-c4cccc(O)c4)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.OC=1C=C(C=CC1)B(O)O>>COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=CC=C2)O)C(=O)O)C=C1OC
C[O:22][C:20]([c:19]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:26]([O:27][CH3:28])[cH:25][c:24]32)[s:23]1)=[O:21].OB(O)[c:12]1[cH:13][cH:14][cH:15][c:16]([OH:17])[cH:18]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][cH:15][c:16]([OH:17])[cH:1...
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccc(O)c1
COc1cc2ncn(-c3nc(-c4cccc(O)c4)c(C(=O)O)s3)c2cc1OC
null
null
null
C-C Coupling
OtherReaction
f263884194c3689072b842d9444db2ca155af322288a9afe28e6da9e83653e3c
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]>>[O;D1;H0:7]=[C:6](-[OH;D1;+0:8])-[c:5]1:[#16;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]
6
[{"value": 6.0, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=CC=C2)O)C(=O)O)C=C1OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 6.0, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=CC=C2)O)C(=O)O)C=C1OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and 3-hydroxyphenylboronic acid (20.7 mg, 0.15 mmol) gave 2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-(3-hydroxy-phenyl)-thiazole-5-carboxylic acid (2.4 mg, 6%) as a white s...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1cscn1.c1ccccc1
c1cscn1.c1ccccc1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1
HBr.B
null
null
null
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccc(O)c1>>COc1cc2ncn(-c3nc(-c4cccc(O)c4)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d3a109297a274f87aaf18a2099d36500
COc1cc2ncn(-c3nc(-c4ccccc4)c(C(=O)O)s3)c2cc1OC.Nc1ccccc1>>COc1cc2ncn(-c3nc(-c4ccccc4)c(C(=O)Nc4ccccc4)s3)c2cc1OC
NC1=CC=CC=C1.COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=CC=C2)C(=O)O)C=C1OC.C(C)N(C(C)C)CC.CN(C)C(=[N+](C)C)ON1C2=C(C=CC=N2)N=N1.F[P-](F)(F)(F)(F)F>>C1(=CC=CC=C1)NC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC=CC=C2
O[C:19]([c:18]1[c:11](-[c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:31]([O:32][CH3:33])[cH:30][c:29]32)[s:28]1)=[O:20].[NH2:21][c:22]1[cH:23][cH:24][cH:25][cH:26][cH:27]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH...
COc1cc2ncn(-c3nc(-c4ccccc4)c(C(=O)O)s3)c2cc1OC.Nc1ccccc1
COc1cc2ncn(-c3nc(-c4ccccc4)c(C(=O)Nc4ccccc4)s3)c2cc1OC
null
null
CN(C=O)C.C(C)(=O)OCC
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1ccccc1)c1sc(-n2cnc3ccccc32)nc1-c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8].[NH2;D1;+0:9]-[c:10](:[c:11]):[c:12]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:9]-[c:10](:[c:11]):[c:12])-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8]
87.6
[{"value": 86.4, "product": "C1(=CC=CC=C1)NC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC=CC=C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 87.6, "product": "C1(=CC=CC=C1)NC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC=CC=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
5
MINUTE
To a solution of 2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-phenyl-thiazole-5-carboxylic acid (30 mg, 0.075 mmol) in dimethylformamide (1 ml) was added diethylisopropylamine (15.6 μL, 0.09 mmol) and HATU (28.5 mg, 0.075 mmol). The mixture was stirred under ambient temperature for 5 min. Aniline (6.8 μL, 0.075 mmol) was add...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1.c1ccccc1
HO-
CN(C=O)C.C(C)(=O)OCC
null
0.083333
COc1cc2ncn(-c3nc(-c4ccccc4)c(C(=O)O)s3)c2cc1OC.Nc1ccccc1>CN(C=O)C.C(C)(=O)OCC>COc1cc2ncn(-c3nc(-c4ccccc4)c(C(=O)Nc4ccccc4)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ccc8952ed6af4a2db53bf5335c8373ae
CCOC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1>>CCOC(=O)c1sc(-n2cnc3cc(O)c(O)cc32)nc1-c1ccccc1
CSC.B(F)(F)F.C(C)OC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC=CC=C2>>C(C)OC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)O)O)C2=CC=CC=C2
C[O:15][c:14]1[cH:13][c:12]2[n:11][cH:10][n:9](-[c:8]3[s:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[c:21](-[c:22]4[cH:23][cH:24][cH:25][cH:26][cH:27]4)[n:20]3)[c:19]2[cH:18][c:16]1[O:17]C>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[s:7][c:8](-[n:9]2[cH:10][n:11][c:12]3[cH:13][c:14]([OH:15])[c:16]([OH:17])[cH:18][c:19]23)[n:...
CCOC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1
CCOC(=O)c1sc(-n2cnc3cc(O)c(O)cc32)nc1-c1ccccc1
null
null
C(Cl)Cl
Deprotection
OtherReaction
a0f05885bbc65ae2846cad0ac34029941211b2ef3a426958b0c8aa83bb16fe86
9df751cd682ad9d54ed75d7313aaead6a019c5d37ede15c4672866d319b900ff
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
C-[O;H0;D2;+0:1]-[c:2]1:[c:3]:[c:4](:[#7;a:5]):[c:6](:[#7;a:7]):[c:8]:[c:9]:1-[O;H0;D2;+0:10]-C>>[#7;a:5]:[c:4]1:[c:3]:[c:2](-[OH;D1;+0:1]):[c:9](-[OH;D1;+0:10]):[c:8]:[c:6]:1:[#7;a:7]
90.4
[{"value": 90.0, "product": "C(C)OC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)O)O)C2=CC=CC=C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 90.4, "product": "C(C)OC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)O)O)C2=CC=CC=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
40
MINUTE
Boron trifluoride dimethylsulfide (4.1 ml, 39 mmol) was added in multiportions over 5 hrs. to a suspension of 2-(5,6-Dimethoxybenzoimidazol-1-yl)-4-phenylthiazole-5-carboxylic acid ethyl ester (2.04 g, 4.99 mmol) in methylene chloride at RT. The mixture was stirred for an additional 40 mins. Ice water was added. Methyl...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether
Aromatic alcohol.Aromatic alcohol
null
null
c1cscn1.c1ccc2[nH]cnc2c1.c1ccccc1
Other
C(Cl)Cl
null
0.666667
CCOC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1-c1ccccc1>C(Cl)Cl>CCOC(=O)c1sc(-n2cnc3cc(O)c(O)cc32)nc1-c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c131f239de98446eb4a934f1e3e146c9
C=Cc1cccc(B(O)O)c1.COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br>>C=Cc1cccc(-c2nc(-n3cnc4cc(OC)c(OC)cc43)sc2C(=O)O)c1
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.C(=C)C=1C=C(C=CC1)B(O)O>>COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=CC=C2)C=C)C(=O)O)C=C1OC
OB(O)[c:7]1[cH:6][cH:5][cH:4][c:3]([CH:2]=[CH2:1])[cH:29]1.C[O:28][C:26]([c:25]1[c:8](Br)[n:9][c:10](-[n:11]2[cH:12][n:13][c:14]3[cH:15][c:16]([O:17][CH3:18])[c:19]([O:20][CH3:21])[cH:22][c:23]23)[s:24]1)=[O:27]>>[CH2:1]=[CH:2][c:3]1[cH:4][cH:5][cH:6][c:7](-[c:8]2[n:9][c:10](-[n:11]3[cH:12][n:13][c:14]4[cH:15][c:16]([O...
C=Cc1cccc(B(O)O)c1.COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br
C=Cc1cccc(-c2nc(-n3cnc4cc(OC)c(OC)cc43)sc2C(=O)O)c1
null
null
null
C-C Coupling
OtherReaction
f263884194c3689072b842d9444db2ca155af322288a9afe28e6da9e83653e3c
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]-[C:12]=[C;D1;H2:13]):[c:14]:[c:15]>>[C;D1;H2:13]=[C:12]-[c:11]:[c:10]:[c;H0;D3;+0:9](-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[OH;D1;+0:8]):[c:14]:[c:15]
64
[{"value": 64.0, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=CC=C2)C=C)C(=O)O)C=C1OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 63.8, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=CC=C2)C=C)C(=O)O)C=C1OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and 3-vinylphenylboronic acid (22 mg, 0.15 mmol) gave 2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-(3-vinyl-phenyl)-thiazole-5-carboxylic acid (26 mg, 64%) as a white solid. ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1ccccc1.c1cscn1
c1ccccc1.c1cscn1
c1ccccc1.c1cscn1.c1ccc2[nH]cnc2c1
HBr.B
null
null
null
C=Cc1cccc(B(O)O)c1.COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br>>C=Cc1cccc(-c2nc(-n3cnc4cc(OC)c(OC)cc43)sc2C(=O)O)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e933b33566be4a8490467ce7b6bfd579
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cc(Cl)cc(Cl)c1>>COc1cc2ncn(-c3nc(-c4cc(Cl)cc(Cl)c4)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.ClC=1C=C(C=C(C1)Cl)B(O)O>>ClC=1C=C(C=C(C1)Cl)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC
C[O:23][C:21]([c:20]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:27]([O:28][CH3:29])[cH:26][c:25]32)[s:24]1)=[O:22].OB(O)[c:12]1[cH:13][c:14]([Cl:15])[cH:16][c:17]([Cl:18])[cH:19]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][c:14]([Cl:15])[cH:16][c:1...
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cc(Cl)cc(Cl)c1
COc1cc2ncn(-c3nc(-c4cc(Cl)cc(Cl)c4)c(C(=O)O)s3)c2cc1OC
null
null
null
C-C Coupling
OtherReaction
f263884194c3689072b842d9444db2ca155af322288a9afe28e6da9e83653e3c
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]>>[O;D1;H0:7]=[C:6](-[OH;D1;+0:8])-[c:5]1:[#16;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]
51.1
[{"value": 51.0, "product": "ClC=1C=C(C=C(C1)Cl)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 51.1, "product": "ClC=1C=C(C=C(C1)Cl)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and 3,5-dichlorophenylboronic acid (27 mg, 0.15 mmol) gave 4-(3,5-Dichloro-phenyl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid (23 mg, 51%) as a whi...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1cscn1.c1ccccc1
c1cscn1.c1ccccc1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1
HBr.B
null
null
null
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cc(Cl)cc(Cl)c1>>COc1cc2ncn(-c3nc(-c4cc(Cl)cc(Cl)c4)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c124c4e5794b44b4af072d5cc6728dfd
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccc(Br)c1>>COc1cc2ncn(-c3nc(-c4cccc(Br)c4)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.BrC=1C=C(C=CC1)B(O)O>>BrC=1C=C(C=CC1)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC
C[O:22][C:20]([c:19]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:26]([O:27][CH3:28])[cH:25][c:24]32)[s:23]1)=[O:21].OB(O)[c:12]1[cH:13][cH:14][cH:15][c:16]([Br:17])[cH:18]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][cH:15][c:16]([Br:17])[cH:1...
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccc(Br)c1
COc1cc2ncn(-c3nc(-c4cccc(Br)c4)c(C(=O)O)s3)c2cc1OC
null
null
null
C-C Coupling
OtherReaction
f263884194c3689072b842d9444db2ca155af322288a9afe28e6da9e83653e3c
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]>>[O;D1;H0:7]=[C:6](-[OH;D1;+0:8])-[c:5]1:[#16;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]
9
[{"value": 9.0, "product": "BrC=1C=C(C=CC1)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 8.7, "product": "BrC=1C=C(C=CC1)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and 3-bromophenylboronic acid (30 mg, 0.15 mmol) gave 4-(3-Bromo-phenyl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid (4.0 mg, 9%) as a white solid. ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1cscn1.c1ccccc1
c1cscn1.c1ccccc1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1
HBr.B
null
null
null
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccc(Br)c1>>COc1cc2ncn(-c3nc(-c4cccc(Br)c4)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d6bdc22d77c04d9da84b1af804deef63
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccc(C(F)(F)F)c1>>COc1cc2ncn(-c3nc(-c4cccc(C(F)(F)F)c4)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.FC(C=1C=C(C=CC1)B(O)O)(F)F>>COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=CC=C2)C(F)(F)F)C(=O)O)C=C1OC
C[O:25][C:23]([c:22]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:29]([O:30][CH3:31])[cH:28][c:27]32)[s:26]1)=[O:24].OB(O)[c:12]1[cH:13][cH:14][cH:15][c:16]([C:17]([F:18])([F:19])[F:20])[cH:21]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][cH:15...
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccc(C(F)(F)F)c1
COc1cc2ncn(-c3nc(-c4cccc(C(F)(F)F)c4)c(C(=O)O)s3)c2cc1OC
null
null
null
C-C Coupling
OtherReaction
f263884194c3689072b842d9444db2ca155af322288a9afe28e6da9e83653e3c
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]>>[O;D1;H0:7]=[C:6](-[OH;D1;+0:8])-[c:5]1:[#16;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]
58.1
[{"value": 58.0, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=CC=C2)C(F)(F)F)C(=O)O)C=C1OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 58.1, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=CC=C2)C(F)(F)F)C(=O)O)C=C1OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and 3-trifluoromethylphenylboronic acid (28.5 mg, 0.15 mmol) gave 2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-(3-trifluoromethyl-phenyl)-thiazole-5-carboxylic acid (26.1 mg,...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1cscn1.c1ccccc1
c1cscn1.c1ccccc1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1
HBr.B
null
null
null
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1cccc(C(F)(F)F)c1>>COc1cc2ncn(-c3nc(-c4cccc(C(F)(F)F)c4)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-740ec3c68917421da89ffd6a67458490
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccc(C(F)(F)F)c(Cl)c1>>COc1cc2ncn(-c3nc(-c4ccc(C(F)(F)F)c(Cl)c4)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.ClC=1C=C(C=CC1C(F)(F)F)B(O)O>>ClC=1C=C(C=CC1C(F)(F)F)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC
C[O:26][C:24]([c:23]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:30]([O:31][CH3:32])[cH:29][c:28]32)[s:27]1)=[O:25].OB(O)[c:12]1[cH:13][cH:14][c:15]([C:16]([F:17])([F:18])[F:19])[c:20]([Cl:21])[cH:22]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:1...
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccc(C(F)(F)F)c(Cl)c1
COc1cc2ncn(-c3nc(-c4ccc(C(F)(F)F)c(Cl)c4)c(C(=O)O)s3)c2cc1OC
null
null
null
C-C Coupling
OtherReaction
f263884194c3689072b842d9444db2ca155af322288a9afe28e6da9e83653e3c
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]>>[O;D1;H0:7]=[C:6](-[OH;D1;+0:8])-[c:5]1:[#16;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]
16
[{"value": 16.0, "product": "ClC=1C=C(C=CC1C(F)(F)F)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 15.9, "product": "ClC=1C=C(C=CC1C(F)(F)F)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and 3-chloro-4-trifluoromethylphenylboronic acid (33.7 mg, 0.15 mmol) gave 4-(3-Chloro-4-trifluoromethyl-phenyl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxy...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1cscn1.c1ccccc1
c1cscn1.c1ccccc1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1
HBr.B
null
null
null
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccc(C(F)(F)F)c(Cl)c1>>COc1cc2ncn(-c3nc(-c4ccc(C(F)(F)F)c(Cl)c4)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ce2172ac60ee41dc908fb5a9b301b45b
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.Cn1ccc2cc(B(O)O)ccc21>>COc1cc2ncn(-c3nc(-c4ccc5c(ccn5C)c4)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.CN1C=CC2=CC(=CC=C12)B(O)O>>COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C=2C=C3C=CN(C3=CC2)C)C(=O)O)C=C1OC
C[O:25][C:23]([c:22]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:29]([O:30][CH3:31])[cH:28][c:27]32)[s:26]1)=[O:24].OB(O)[c:12]1[cH:13][cH:14][c:15]2[c:16]([cH:17][cH:18][n:19]2[CH3:20])[cH:21]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][c:15...
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.Cn1ccc2cc(B(O)O)ccc21
COc1cc2ncn(-c3nc(-c4ccc5c(ccn5C)c4)c(C(=O)O)s3)c2cc1OC
null
null
null
C-C Coupling
OtherReaction
ceebcf352d77229d3b9c14eff09e7aac88aca94d5d4385b9ea0d401292d74f92
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc2c(c1)ncn2-c1nc(-c2ccc3[nH]ccc3c2)cs1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9]1:[c:10]:[c:11]:[c:12](:[#7;a:13]):[c:14]:[c:15]:1>>[#7;a:13]:[c:12]1:[c:11]:[c:10]:[c;H0;D3;+0:9](-[c;H0;D3;+0:1]2:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:2-[C:6](=[O;D1;H0:7])-[OH;D1;+0:8]):[c:15]:[c:14]:1
12
[{"value": 12.0, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C=2C=C3C=CN(C3=CC2)C)C(=O)O)C=C1OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 11.7, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C=2C=C3C=CN(C3=CC2)C)C(=O)O)C=C1OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and N-methylindole-5-boronic acid (26.2 mg, 0.15 mmol) gave 2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-(1-methyl-1H-indol-5-yl)-thiazole-5-carboxylic acid (5.1 mg, 12%) as ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1cscn1.c1ccc2[nH]ccc2c1
c1cscn1.c1ccc2[nH]ccc2c1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccc2[nH]ccc2c1
HBr.B
null
null
null
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.Cn1ccc2cc(B(O)O)ccc21>>COc1cc2ncn(-c3nc(-c4ccc5c(ccn5C)c4)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-38f139cc1fb6484eb8bbcda09d1148c6
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccc(F)c(F)c1>>COc1cc2ncn(-c3nc(-c4ccc(F)c(F)c4)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.FC=1C=C(C=CC1F)B(O)O>>FC=1C=C(C=CC1F)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC
C[O:23][C:21]([c:20]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:27]([O:28][CH3:29])[cH:26][c:25]32)[s:24]1)=[O:22].OB(O)[c:12]1[cH:13][cH:14][c:15]([F:16])[c:17]([F:18])[cH:19]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][c:15]([F:16])[c:17](...
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccc(F)c(F)c1
COc1cc2ncn(-c3nc(-c4ccc(F)c(F)c4)c(C(=O)O)s3)c2cc1OC
null
null
null
C-C Coupling
OtherReaction
f263884194c3689072b842d9444db2ca155af322288a9afe28e6da9e83653e3c
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]>>[O;D1;H0:7]=[C:6](-[OH;D1;+0:8])-[c:5]1:[#16;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]
21
[{"value": 21.0, "product": "FC=1C=C(C=CC1F)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 20.8, "product": "FC=1C=C(C=CC1F)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and 3,4-difluorophenylboronic acid (23.7 mg, 0.15 mmol) gave 4-(3,4-Difluoro-phenyl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid (8.7 mg, 21%) as a ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1cscn1.c1ccccc1
c1cscn1.c1ccccc1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1
HBr.B
null
null
null
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccc(F)c(F)c1>>COc1cc2ncn(-c3nc(-c4ccc(F)c(F)c4)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e85216952b934b1c8df0c3f4ada64753
CCOC(=O)c1sc(-n2cnc3cc(O)c(O)cc32)nc1-c1ccccc1.CN1CCCC1=O.COCCBr>>COCCOc1cc2ncn(-c3nc(-c4ccccc4)c(C(=O)O)s3)c2cc1OCCOC
O.C(C)OC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)O)O)C2=CC=CC=C2.COCCBr.C([O-])([O-])=O.[K+].[K+].CN1C(CCC1)=O>>COCCOC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=CC=C2)C(=O)O)C=C1OCCOC
[CH3:3][CH2:4][O:24][C:22]([c:21]1[c:14](-[c:15]2[cH:16][cH:17][cH:18][cH:19][cH:20]2)[n:13][c:12](-[n:11]2[cH:10][n:9][c:8]3[cH:7][c:6]([OH:5])[c:28]([OH:29])[cH:27][c:26]32)[s:25]1)=[O:23].O=C1CCCN1[CH3:1].Br[CH2:30][CH2:31][O:32][CH3:33]>>[CH3:1][O:2][CH2:3][CH2:4][O:5][c:6]1[cH:7][c:8]2[n:9][cH:10][n:11](-[c:12]3[n...
CCOC(=O)c1sc(-n2cnc3cc(O)c(O)cc32)nc1-c1ccccc1.CN1CCCC1=O.COCCBr
COCCOc1cc2ncn(-c3nc(-c4ccccc4)c(C(=O)O)s3)c2cc1OCCOC
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
1f9d7dda6aa554619ebd2cce26e6d436fea7d5187b4ebc73c49c366581561a06
31b20b6e5ca29276309667336e59ba1c90635c7dc1b4092b9a2f6410a6a41368
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Br-[CH2;D2;+0:1]-[C:2]-[#8:3].O=C1-C-C-C-N-1-[CH3;D1;+0:4].[#16;a:5]:[c:6](-[C:7](=[O;D1;H0:8])-[O;H0;D2;+0:9]-[CH2;D2;+0:10]-[CH3;D1;+0:11]):[c:12]:[#7;a:13].[#7;a:14]:[c:15]1:[c:16]:[c:17](-[OH;D1;+0:18]):[c:19](-[OH;D1;+0:20]):[c:21]:[c:22]:1:[#7;a:23]>>[#16;a:5]:[c:6](-[C:7](=[O;D1;H0:8])-[OH;D1;+0:9]):[c:12]:[#7;a...
17
[{"value": 17.0, "product": "COCCOC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=CC=C2)C(=O)O)C=C1OCCOC", "details": "PERCENTYIELD", "is_desired": false}]
80
CELSIUS
4
HOUR
A mixture of 2-(5,6-dihydroxy-benzoimidazol-1-yl)-4-phenyl-thiazole-5-carboxylic acid ethyl ester (118.8 mg, 0.31 mmol, intermediate for Example 39), bromoethyl methyl ether (0.1 ml) and potassium carbonate (200 mg) in N-methylpyrrolidone (2 ml) was stirred at RT overnight and 80° C. for 4 hr. Water was added, and the ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester.Tertiary amide.Aromatic alcohol.Aromatic alcohol
Carboxylic acid.Ether.Ether.Ether
C1CCNC1
null
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1
HBr
null
80
4
CCOC(=O)c1sc(-n2cnc3cc(O)c(O)cc32)nc1-c1ccccc1.CN1CCCC1=O.COCCBr>>COCCOc1cc2ncn(-c3nc(-c4ccccc4)c(C(=O)O)s3)c2cc1OCCOC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1f7f72c44f7944dca4c7b3ae939ee678
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OCc1cccc(B(O)O)c1>>COc1cc2ncn(-c3nc(-c4cccc(CO)c4)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.OCC=1C=C(C=CC1)B(O)O>>COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=CC=C2)CO)C(=O)O)C=C1OC
C[O:23][C:21]([c:20]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:27]([O:28][CH3:29])[cH:26][c:25]32)[s:24]1)=[O:22].OB(O)[c:12]1[cH:13][cH:14][cH:15][c:16]([CH2:17][OH:18])[cH:19]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][cH:15][c:16]([CH2:...
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OCc1cccc(B(O)O)c1
COc1cc2ncn(-c3nc(-c4cccc(CO)c4)c(C(=O)O)s3)c2cc1OC
null
null
null
C-C Coupling
OtherReaction
f263884194c3689072b842d9444db2ca155af322288a9afe28e6da9e83653e3c
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]>>[O;D1;H0:7]=[C:6](-[OH;D1;+0:8])-[c:5]1:[#16;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]
2
[{"value": 2.0, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=CC=C2)CO)C(=O)O)C=C1OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 1.9, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=CC=C2)CO)C(=O)O)C=C1OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and 3-hydroxymethylphenylboronic acid (22.9 mg, 0.15 mmol) gave 2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-(3-hydroxymethyl-phenyl)-thiazole-5-carboxylic acid (0.8 mg, 2.0%...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1cscn1.c1ccccc1
c1cscn1.c1ccccc1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1
HBr.B
null
null
null
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OCc1cccc(B(O)O)c1>>COc1cc2ncn(-c3nc(-c4cccc(CO)c4)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b5b66d178564491d9f7645ea0d9be57e
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccc2c(c1)OCCO2>>COc1cc2ncn(-c3nc(-c4ccc5c(c4)OCCO5)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.O1CCOC2=C1C=CC(=C2)B(O)O>>O1CCOC2=C1C=CC(=C2)C=2N=C(SC2C(=O)O)N2C=NC1=C2C=C(C(=C1)OC)OC
C[O:25][C:23]([c:22]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:29]([O:30][CH3:31])[cH:28][c:27]32)[s:26]1)=[O:24].OB(O)[c:12]1[cH:13][cH:14][c:15]2[c:16]([cH:17]1)[O:18][CH2:19][CH2:20][O:21]2>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][c:15...
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccc2c(c1)OCCO2
COc1cc2ncn(-c3nc(-c4ccc5c(c4)OCCO5)c(C(=O)O)s3)c2cc1OC
null
null
null
C-C Coupling
OtherReaction
f589e70e63409b9e35e63fa7758e87bfecd59dc704f8541cd1578b3741023d3c
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc2c(c1)ncn2-c1nc(-c2ccc3c(c2)OCCO3)cs1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]-[#8:14]>>[#8:14]-[c:13]:[c:12]:[c;H0;D3;+0:9](-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[OH;D1;+0:8]):[c:10]:[c:11]
22
[{"value": 22.0, "product": "O1CCOC2=C1C=CC(=C2)C=2N=C(SC2C(=O)O)N2C=NC1=C2C=C(C(=C1)OC)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 21.6, "product": "O1CCOC2=C1C=CC(=C2)C=2N=C(SC2C(=O)O)N2C=NC1=C2C=C(C(=C1)OC)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and 1,4-benzodioxane-6-boronic acid (27 mg, 0.15 mmol) gave 4-(2,3-Dihydro-benzo[1,4]dioxin-6-yl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid (9.5 m...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1cscn1.c1ccc2c(c1)OCCO2
c1cscn1.c1ccc2c(c1)OCCO2
c1ccc2[nH]cnc2c1.c1cscn1.c1ccc2c(c1)OCCO2
HBr.B
null
null
null
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)c1ccc2c(c1)OCCO2>>COc1cc2ncn(-c3nc(-c4ccc5c(c4)OCCO5)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2601f61c18774ab7a121314b7e5cdd18
C=Cc1ccc(B(O)O)cc1.COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br>>C=Cc1ccc(-c2nc(-n3cnc4cc(OC)c(OC)cc43)sc2C(=O)O)cc1
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.B(C1=CC=C(C=C1)C=C)(O)O>>COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=C(C=C2)C=C)C(=O)O)C=C1OC
OB(O)[c:6]1[cH:5][cH:4][c:3]([CH:2]=[CH2:1])[cH:29][cH:28]1.C[O:27][C:25]([c:24]1[c:7](Br)[n:8][c:9](-[n:10]2[cH:11][n:12][c:13]3[cH:14][c:15]([O:16][CH3:17])[c:18]([O:19][CH3:20])[cH:21][c:22]23)[s:23]1)=[O:26]>>[CH2:1]=[CH:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[n:8][c:9](-[n:10]3[cH:11][n:12][c:13]4[cH:14][c:15]([O:16][CH...
C=Cc1ccc(B(O)O)cc1.COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br
C=Cc1ccc(-c2nc(-n3cnc4cc(OC)c(OC)cc43)sc2C(=O)O)cc1
null
null
null
C-C Coupling
OtherReaction
f263884194c3689072b842d9444db2ca155af322288a9afe28e6da9e83653e3c
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]>>[O;D1;H0:7]=[C:6](-[OH;D1;+0:8])-[c:5]1:[#16;a:4]:[c:3]:[#7;a:2]:[c;H0;D3;+0:1]:1-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]
37.3
[{"value": 37.0, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=C(C=C2)C=C)C(=O)O)C=C1OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 37.3, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC=C(C=C2)C=C)C(=O)O)C=C1OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and 4-vinylboronic acid (22.2 mg, 0.15 mmol) gave 2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-(4-vinyl-phenyl)-thiazole-5-carboxylic acid (15.2 mg, 37%) as a white solid. 1H...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1ccccc1.c1cscn1
c1ccccc1.c1cscn1
c1ccccc1.c1cscn1.c1ccc2[nH]cnc2c1
HBr.B
null
null
null
C=Cc1ccc(B(O)O)cc1.COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br>>C=Cc1ccc(-c2nc(-n3cnc4cc(OC)c(OC)cc43)sc2C(=O)O)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-84897f4b243f4ede9a0f4e007c56cd65
CN(C)C(=O)c1cccc(B(O)O)c1.COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br>>COc1cc2ncn(-c3nc(-c4cccc(C(=O)N(C)C)c4)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.CN(C(=O)C=1C=C(C=CC1)B(O)O)C>>COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=CC=C2)C(N(C)C)=O)C(=O)O)C=C1OC
OB(O)[c:12]1[cH:13][cH:14][cH:15][c:16]([C:17](=[O:18])[N:19]([CH3:20])[CH3:21])[cH:22]1.C[O:26][C:24]([c:23]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:30]([O:31][CH3:32])[cH:29][c:28]32)[s:27]1)=[O:25]>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][c...
CN(C)C(=O)c1cccc(B(O)O)c1.COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br
COc1cc2ncn(-c3nc(-c4cccc(C(=O)N(C)C)c4)c(C(=O)O)s3)c2cc1OC
null
null
null
C-C Coupling
OtherReaction
f263884194c3689072b842d9444db2ca155af322288a9afe28e6da9e83653e3c
5af41468c321f267448297a8abdded64f3cc5543e523be88c60c8574c327b358
c1ccc(-c2csc(-n3cnc4ccccc43)n2)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]-[C:14](-[#7:15])=[O;D1;H0:16]>>[#7:15]-[C:14](=[O;D1;H0:16])-[c:13]:[c:12]:[c;H0;D3;+0:9](-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[OH;D1;+0:8]):[c:1...
4
[{"value": 4.0, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=CC=C2)C(N(C)C)=O)C(=O)O)C=C1OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 4.0, "product": "COC1=CC2=C(N(C=N2)C=2SC(=C(N2)C2=CC(=CC=C2)C(N(C)C)=O)C(=O)O)C=C1OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (40 mg, 0.1 mmol) and 3-dimethylcarbamoylphenylboronic acid (29 mg, 0.15 mmol) gave 2-(5,6-Dimethoxy-benzoimidazol-1-yl)-4-(3-dimethylcarbamoyl-phenyl)-thiazole-5-carboxylic acid (1.8 mg...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Boronic acid
Carboxylic acid
c1ccccc1.c1cscn1
c1cscn1.c1ccccc1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1
HBr.B
null
null
null
CN(C)C(=O)c1cccc(B(O)O)c1.COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br>>COc1cc2ncn(-c3nc(-c4cccc(C(=O)N(C)C)c4)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-79c97d7eb5cf42ed9c08b38a0ff2f9fc
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC.NNC(=O)c1cccs1>>COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)NNC(=O)c4cccs4)s3)c2cc1OC
ClC=1C=C(C=CC1)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC.S1C(=CC=C1)C(=O)NN.CN(C)C(=[N+](C)C)ON1C2=C(C=CC=N2)N=N1.F[P-](F)(F)(F)(F)F.C(C)(C)N(CC)C(C)C>>ClC=1C=C(C=CC1)C=1N=C(SC1C(=O)NNC(=O)C=1SC=CC1)N1C=NC2=C1C=C(C(=C2)OC)OC
O[C:20]([c:19]1[c:11](-[c:12]2[cH:13][cH:14][cH:15][c:16]([Cl:17])[cH:18]2)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:34]([O:35][CH3:36])[cH:33][c:32]32)[s:31]1)=[O:21].[NH2:22][NH:23][C:24](=[O:25])[c:26]1[cH:27][cH:28][cH:29][s:30]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:...
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC.NNC(=O)c1cccs1
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)NNC(=O)c4cccs4)s3)c2cc1OC
null
null
O.CN(C=O)C
Acylation
Carboxylic acid with primary amine to amide
1bfc5046b360bb38c235d234cdd252f03d34a0792ef57a2cdb032482310d9689
1f93e2b4a6ed796a4645f0486672499ca332a9bc5c180e504c9a46d8eb8d844d
O=C(NNC(=O)c1sc(-n2cnc3ccccc32)nc1-c1ccccc1)c1cccs1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8].[#16;a:9]:[c:10]-[C:11](=[O;D1;H0:12])-[#7:13]-[NH2;D1;+0:14]>>[#16;a:9]:[c:10]-[C:11](=[O;D1;H0:12])-[#7:13]-[NH;D2;+0:14]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8]
70.2
[{"value": 70.2, "product": "ClC=1C=C(C=CC1)C=1N=C(SC1C(=O)NNC(=O)C=1SC=CC1)N1C=NC2=C1C=C(C(=C2)OC)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 70.2, "product": "ClC=1C=C(C=CC1)C=1N=C(SC1C(=O)NNC(=O)C=1SC=CC1)N1C=NC2=C1C=C(C(=C2)OC)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To a solution of 4-(3-Chloro-phenyl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid (41 mg, 0.1 mmol) and thiophene-2-carboxylic acid hydrazide (14.2 mg, 0.1 mmol, Aldrich) in N,N-dimethylformamide (1 ml) was added HATU (38 mg, 0.1 mmol) and diisopropylethylamine (26 μl, 0.15 mmol). The mixture was sti...
10.6084/m9.figshare.5104873.v1
null
Acylhydrazine.Carboxylic acid
Acylhydrazine.Acylhydrazine
null
null
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1.c1ccsc1
HO-
O.CN(C=O)C
null
8
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC.NNC(=O)c1cccs1>O.CN(C=O)C>COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)NNC(=O)c4cccs4)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-fb4584ffdf00451db8c31b4290fac671
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC.Nc1ccncn1>>COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)Nc4ccncn4)s3)c2cc1OC
ClC=1C=C(C=CC1)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC.NC1=NC=NC=C1>>N1=CN=C(C=C1)NC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC(=CC=C2)Cl
O[C:20]([c:19]1[c:11](-[c:12]2[cH:13][cH:14][cH:15][c:16]([Cl:17])[cH:18]2)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:32]([O:33][CH3:34])[cH:31][c:30]32)[s:29]1)=[O:21].[NH2:22][c:23]1[cH:24][cH:25][n:26][cH:27][n:28]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:...
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC.Nc1ccncn1
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)Nc4ccncn4)s3)c2cc1OC
null
null
null
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1ccncn1)c1sc(-n2cnc3ccccc32)nc1-c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8].[NH2;D1;+0:9]-[c:10]1:[#7;a:11]:[c:12]:[#7;a:13]:[c:14]:[c:15]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:9]-[c:10]1:[#7;a:11]:[c:12]:[#7;a:13]:[c:14]:[c:15]:1)-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8]
69.7
[{"value": 69.7, "product": "N1=CN=C(C=C1)NC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC(=CC=C2)Cl", "details": "PERCENTYIELD", "is_desired": false}, {"value": 69.6, "product": "N1=CN=C(C=C1)NC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC(=CC=C2)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 53, 4-(3-Chloro-phenyl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid (41 mg, 0.1 mmol) and 4-aminopyrimidine (9.5 mg, 0.1 mmol, Aldrich) gave 4-(3-Chloro-phenyl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid pyrimidin-4-ylamide (34.3 mg, ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1.c1cncnc1
HO-
null
null
null
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC.Nc1ccncn1>>COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)Nc4ccncn4)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e6b268bfd146479a94fd857e3d4e9c59
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC.COc1cccc(N)c1>>COc1cccc(NC(=O)c2sc(-n3cnc4cc(OC)c(OC)cc43)nc2-c2cccc(Cl)c2)c1
ClC=1C=C(C=CC1)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC.COC1=CC(=CC=C1)N>>COC=1C=C(C=CC1)NC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC(=CC=C2)Cl
O[C:9](=[O:10])[c:11]1[s:12][c:13](-[n:14]2[cH:15][n:16][c:17]3[cH:18][c:19]([O:20][CH3:21])[c:22]([O:23][CH3:24])[cH:25][c:26]23)[n:27][c:28]1-[c:29]1[cH:30][cH:31][cH:32][c:33]([Cl:34])[cH:35]1.[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7]([NH2:8])[cH:36]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7]([NH:8][C:9](=[O:10])[c...
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC.COc1cccc(N)c1
COc1cccc(NC(=O)c2sc(-n3cnc4cc(OC)c(OC)cc43)nc2-c2cccc(Cl)c2)c1
null
null
null
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1ccccc1)c1sc(-n2cnc3ccccc32)nc1-c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8].[NH2;D1;+0:9]-[c:10](:[c:11]):[c:12]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:9]-[c:10](:[c:11]):[c:12])-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8]
86.6
[{"value": 86.6, "product": "COC=1C=C(C=CC1)NC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC(=CC=C2)Cl", "details": "PERCENTYIELD", "is_desired": false}, {"value": 86.6, "product": "COC=1C=C(C=CC1)NC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC(=CC=C2)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 53, 4-(3-Chloro-phenyl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid (41 mg, 0.1 mmol) and 3-anisidine (12.3 mg, 0.1 mmol, Aldrich) gave 4-(3-Chloro-phenyl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid (3-methoxy-phenyl)-amide (45.1 mg, ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.c1cscn1.c1ccc2[nH]cnc2c1.c1ccccc1
HO-
null
null
null
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC.COc1cccc(N)c1>>COc1cccc(NC(=O)c2sc(-n3cnc4cc(OC)c(OC)cc43)nc2-c2cccc(Cl)c2)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-dcf8546ca9be4051a5b5f5b06fbb71f0
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC.Nc1nccs1>>COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)Nc4nccs4)s3)c2cc1OC
ClC=1C=C(C=CC1)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC.NC=1SC=CN1>>S1C(=NC=C1)NC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC(=CC=C2)Cl
O[C:20]([c:19]1[c:11](-[c:12]2[cH:13][cH:14][cH:15][c:16]([Cl:17])[cH:18]2)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:31]([O:32][CH3:33])[cH:30][c:29]32)[s:28]1)=[O:21].[NH2:22][c:23]1[n:24][cH:25][cH:26][s:27]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:...
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC.Nc1nccs1
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)Nc4nccs4)s3)c2cc1OC
null
null
null
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1nccs1)c1sc(-n2cnc3ccccc32)nc1-c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8].[NH2;D1;+0:9]-[c:10]1:[#16;a:11]:[c:12]:[c:13]:[#7;a:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:9]-[c:10]1:[#16;a:11]:[c:12]:[c:13]:[#7;a:14]:1)-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8]
79.5
[{"value": 79.5, "product": "S1C(=NC=C1)NC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC(=CC=C2)Cl", "details": "PERCENTYIELD", "is_desired": false}, {"value": 79.5, "product": "S1C(=NC=C1)NC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC(=CC=C2)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 53, 4-(3-Chloro-phenyl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid (41 mg, 0.1 mmol) and 2-aminothiazole (10.0 mg, 0.1 mmol, Aldrich) gave 4-(3-Chloro-phenyl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid thiazol-2-ylamide (39.6 mg, 79....
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1.c1cscn1
HO-
null
null
null
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC.Nc1nccs1>>COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)Nc4nccs4)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-bfc0ee7048484136b0ef09ad3b98be1b
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC.Nn1cnnc1>>COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)Nn4cnnc4)s3)c2cc1OC
ClC=1C=C(C=CC1)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC.NN1C=NN=C1>>N=1N=CN(C1)NC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC(=CC=C2)Cl
O[C:20]([c:19]1[c:11](-[c:12]2[cH:13][cH:14][cH:15][c:16]([Cl:17])[cH:18]2)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:31]([O:32][CH3:33])[cH:30][c:29]32)[s:28]1)=[O:21].[NH2:22][n:23]1[cH:24][n:25][n:26][cH:27]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:...
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC.Nn1cnnc1
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)Nn4cnnc4)s3)c2cc1OC
null
null
null
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nn1cnnc1)c1sc(-n2cnc3ccccc32)nc1-c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8].[NH2;D1;+0:9]-[#7;a:10]1:[c:11]:[#7;a:12]:[#7;a:13]:[c:14]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:9]-[#7;a:10]1:[c:11]:[#7;a:12]:[#7;a:13]:[c:14]:1)-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8]
5
[{"value": 5.0, "product": "N=1N=CN(C1)NC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC(=CC=C2)Cl", "details": "PERCENTYIELD", "is_desired": false}, {"value": 5.0, "product": "N=1N=CN(C1)NC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC(=CC=C2)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 53, 4-(3-Chloro-phenyl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid (41 mg, 0.1 mmol) and 4-amino-1,2,4-triazole (8.4 mg, 0.1 mmol, Aldrich) gave 4-(3-Chloro-phenyl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid [1,2,4]triazol-4-ylamide ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1.c1nnc[nH]1
HO-
null
null
null
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC.Nn1cnnc1>>COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)Nn4cnnc4)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a9b9f7be58f945379c7e2def803e8dae
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC.Cc1cccc(C(=O)NN)c1>>COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)NNC(=O)c4cccc(C)c4)s3)c2cc1OC
ClC=1C=C(C=CC1)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC.C1(=CC(=CC=C1)C(=O)NN)C>>ClC=1C=C(C=CC1)C=1N=C(SC1C(=O)NNC(C1=CC(=CC=C1)C)=O)N1C=NC2=C1C=C(C(=C2)OC)OC
O[C:20]([c:19]1[c:11](-[c:12]2[cH:13][cH:14][cH:15][c:16]([Cl:17])[cH:18]2)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:36]([O:37][CH3:38])[cH:35][c:34]32)[s:33]1)=[O:21].[NH2:22][NH:23][C:24](=[O:25])[c:26]1[cH:27][cH:28][cH:29][c:30]([CH3:31])[cH:32]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8]...
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC.Cc1cccc(C(=O)NN)c1
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)NNC(=O)c4cccc(C)c4)s3)c2cc1OC
null
null
null
Acylation
Carboxylic acid with primary amine to amide
1bfc5046b360bb38c235d234cdd252f03d34a0792ef57a2cdb032482310d9689
1f93e2b4a6ed796a4645f0486672499ca332a9bc5c180e504c9a46d8eb8d844d
O=C(NNC(=O)c1sc(-n2cnc3ccccc32)nc1-c1ccccc1)c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8].[NH2;D1;+0:9]-[#7:10]-[C:11](=[O;D1;H0:12])-[c:13]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:9]-[#7:10]-[C:11](=[O;D1;H0:12])-[c:13])-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8]
3.8
[{"value": 3.8, "product": "ClC=1C=C(C=CC1)C=1N=C(SC1C(=O)NNC(C1=CC(=CC=C1)C)=O)N1C=NC2=C1C=C(C(=C2)OC)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 3.8, "product": "ClC=1C=C(C=CC1)C=1N=C(SC1C(=O)NNC(C1=CC(=CC=C1)C)=O)N1C=NC2=C1C=C(C(=C2)OC)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false...
null
null
null
null
In a similar manner as described for Example 53, 4-(3-Chloro-phenyl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid (41 mg, 0.1 mmol) and m-toluic acid hydrazide (15.0 mg, 0.1 mmol, Lancaster) gave 3-Methyl-benzoic acid N′-[4-(3-chloro-phenyl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carbonyl]-h...
10.6084/m9.figshare.5104873.v1
null
Acylhydrazine.Carboxylic acid
Acylhydrazine.Acylhydrazine
null
null
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1.c1ccccc1
HO-
null
null
null
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC.Cc1cccc(C(=O)NN)c1>>COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)NNC(=O)c4cccc(C)c4)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-cdfd204a5bc24d5ca42307623e861556
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC.Nc1cc[nH]c(=O)n1>>COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)Nc4cc[nH]c(=O)n4)s3)c2cc1OC
ClC=1C=C(C=CC1)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC.N1C(=O)N=C(N)C=C1>>O=C1NC=CC(=N1)NC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC(=CC=C2)Cl
O[C:20]([c:19]1[c:11](-[c:12]2[cH:13][cH:14][cH:15][c:16]([Cl:17])[cH:18]2)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:33]([O:34][CH3:35])[cH:32][c:31]32)[s:30]1)=[O:21].[NH2:22][c:23]1[cH:24][cH:25][nH:26][c:27](=[O:28])[n:29]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c...
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC.Nc1cc[nH]c(=O)n1
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)Nc4cc[nH]c(=O)n4)s3)c2cc1OC
null
null
null
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1cc[nH]c(=O)n1)c1sc(-n2cnc3ccccc32)nc1-c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8].[NH2;D1;+0:9]-[c:10]1:[#7;a:11]:[c:12]:[#7;a:13]:[c:14]:[c:15]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:9]-[c:10]1:[#7;a:11]:[c:12]:[#7;a:13]:[c:14]:[c:15]:1)-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[c:8]
11
[{"value": 11.0, "product": "O=C1NC=CC(=N1)NC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC(=CC=C2)Cl", "details": "PERCENTYIELD", "is_desired": false}, {"value": 11.0, "product": "O=C1NC=CC(=N1)NC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)C2=CC(=CC=C2)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 53, 4-(3-Chloro-phenyl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid (41 mg, 0.1 mmol) and cytosine (11.1 mg, 0.1 mmol, Aldrich) gave 4-(3-Chloro-phenyl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid (2-oxo-1,2-dihydro-pyrimidin-4-yl)-ami...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccc2[nH]cnc2c1.c1cscn1.c1ccccc1.c1ccncn1
HO-
null
null
null
COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)O)s3)c2cc1OC.Nc1cc[nH]c(=O)n1>>COc1cc2ncn(-c3nc(-c4cccc(Cl)c4)c(C(=O)Nc4cc[nH]c(=O)n4)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-99e207888bd243beabf304f07f498f58
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)C1(Cl)C=CC=CN1>>COc1cc2ncn(-c3nc(-c4ccnc(Cl)c4)c(C(=O)O)s3)c2cc1OC
COC(=O)C1=C(N=C(S1)N1C=NC2=C1C=C(C(=C2)OC)OC)Br.ClC1(NC=CC=C1)B(O)O>>ClC1=NC=CC(=C1)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC
C[O:22][C:20]([c:19]1[c:11](Br)[n:10][c:9](-[n:8]2[cH:7][n:6][c:5]3[cH:4][c:3]([O:2][CH3:1])[c:26]([O:27][CH3:28])[cH:25][c:24]32)[s:23]1)=[O:21].OB(O)[C:16]1([Cl:17])[NH:15][CH:14]=[CH:13][CH:12]=[CH:18]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8](-[c:9]3[n:10][c:11](-[c:12]4[cH:13][cH:14][n:15][c:16]([Cl:17])[cH...
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)C1(Cl)C=CC=CN1
COc1cc2ncn(-c3nc(-c4ccnc(Cl)c4)c(C(=O)O)s3)c2cc1OC
null
null
null
C-C Coupling
OtherReaction
48bc47ed9a4b0545686f380853b2598405ea077723a76e78c487ad11a319ba9c
05e3eb4ca364d4dd5d7d9c0848a2b8e41d59224ac4a93bb541e406c3ea7919ef
c1ccc2c(c1)ncn2-c1nc(-c2ccncc2)cs1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:1-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-C.O-B(-O)-[C;H0;D4;+0:9]1(-[Cl;D1;H0:10])-[CH;D2;+0:11]=[CH;D2;+0:12]-[CH;D2;+0:13]=[CH;D2;+0:14]-[NH;D2;+0:15]-1>>[Cl;D1;H0:10]-[c;H0;D3;+0:9]1:[cH;D2;+0:11]:[c;H0;D3;+0:12](-[c;H0;D3;+0:1]2:[#7;a:2]:[c:3]:[#16;a:4]:[c:5]:2-[C:6](=[...
46.4
[{"value": 46.4, "product": "ClC1=NC=CC(=C1)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 46.4, "product": "ClC1=NC=CC(=C1)C=1N=C(SC1C(=O)O)N1C=NC2=C1C=C(C(=C2)OC)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
In a similar manner as described for Example 26, 4-bromo-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid methyl ester (120 mg, 0.3 mmol) and 2-chloropyridine-2-boronic acid (71 mg, 0.45 mmol) gave 4-(2-Chloro-pyridin-4-yl)-2-(5,6-dimethoxy-benzoimidazol-1-yl)-thiazole-5-carboxylic acid (58 mg, 46.4%) as...
10.6084/m9.figshare.5104873.v1
null
Enamine.Aromatic halide.Tertiary halide.Ester.Boronic acid.Conjugated diene
Aromatic halide.Carboxylic acid
c1cscn1.C1=CCNC=C1
c1cscn1.c1ccncc1
c1ccc2[nH]cnc2c1.c1cscn1.c1ccncc1
HBr.B
null
null
null
COC(=O)c1sc(-n2cnc3cc(OC)c(OC)cc32)nc1Br.OB(O)C1(Cl)C=CC=CN1>>COc1cc2ncn(-c3nc(-c4ccnc(Cl)c4)c(C(=O)O)s3)c2cc1OC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8c87d20b662440d4a55bb0bd3cc07d10
O=C(OO)c1cccc(Cl)c1>>CC1(C)OC(=O)COC1=O
ClC1=CC(=CC=C1)C(=O)OO>>CC1(OC(COC1=O)=O)C
Cl[c:5]1[cH:3][c:2]([C:9]([O:8][OH:4])=[O:10])[cH:1]c[cH:7]1>>[CH3:1][C:2]1([CH3:3])[O:4][C:5](=[O:6])[CH2:7][O:8][C:9]1=[O:10]
O=C(OO)c1cccc(Cl)c1
CC1(C)OC(=O)COC1=O
null
null
ClCCl
Miscellaneous
OtherReaction
4400727cd1198764fe8b1969daa817e812a15f25c8b234ac111afebd28f75e4d
08ae86020599855ef67800c69886dbf7915f83dafbd43cf0edc5db86fcf85ed8
O=C1COC(=O)CO1
Cl-[c;H0;D3;+0:1]1:[cH;D2;+0:2]:[c;H0;D3;+0:3](-[C:4](=[O;D1;H0:5])-[O;H0;D2;+0:6]-[OH;D1;+0:7]):[cH;D2;+0:8]:c:[cH;D2;+0:9]:1>>[CH3;D1;+0:8]-[C;H0;D4;+0:3]1(-[CH3;D1;+0:2])-[O;H0;D2;+0:7]-[C;H0;D3;+0:1](=[O;D1;H0:10])-[CH2;D2;+0:9]-[O;H0;D2;+0:6]-[C:4]-1=[O;D1;H0:5]
null
[]
-18
CELSIUS
null
null
A solution of 5 g of cyclic keto-ester (39 mmol) and 8.1 g of metachloroperbenzoic acid (1.2 eq.) in 40 ml of dichloromethane is heated under reflux for 24 hours. The complete conversion of the ring with 5 members is monitored by NMR 1H on a sample. The reaction medium is then cooled down to −18° C. overnight then filt...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Peroxide
Ester.Ester
c1ccccc1
C1COCCO1
C1COCCO1
Other
ClCCl
-18
null
O=C(OO)c1cccc(Cl)c1>ClCCl>CC1(C)OC(=O)COC1=O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-888d8d47fb5c4f5f9649e35e4e8651bf
O=C(OO)c1cccc(Cl)c1.O=S(=O)(O)C(F)(F)F>>CC1(C)OC(=O)COC1=O
ClC1=CC(=CC=C1)C(=O)OO.FC(S(=O)(=O)O)(F)F>>CC1(OC(COC1=O)=O)C
Clc1[cH:3][c:2]([C:9]([O:8][OH:4])=[O:10])[cH:1]c[cH:7]1.O=S(O)([C:5](F)(F)F)=[O:6]>>[CH3:1][C:2]1([CH3:3])[O:4][C:5](=[O:6])[CH2:7][O:8][C:9]1=[O:10]
O=C(OO)c1cccc(Cl)c1.O=S(=O)(O)C(F)(F)F
CC1(C)OC(=O)COC1=O
null
null
ClCCl
Heteroatom Alkylation and Arylation
OtherReaction
03f692efa2fbafa3dc3b5ecb485e08b376972c9c82d2ceb92cfd883696edd565
311d7bfa1bd9b6b7c60384461a4bc313a1f774cce7ab37764991ad07ffb60024
O=C1COC(=O)CO1
Cl-c1:[cH;D2;+0:1]:[c;H0;D3;+0:2](-[C:3](=[O;D1;H0:4])-[O;H0;D2;+0:5]-[OH;D1;+0:6]):[cH;D2;+0:7]:c:[cH;D2;+0:8]:1.F-[C;H0;D4;+0:9](-F)(-F)-S(-O)(=O)=[O;H0;D1;+0:10]>>[CH3;D1;+0:7]-[C;H0;D4;+0:2]1(-[CH3;D1;+0:1])-[O;H0;D2;+0:6]-[C;H0;D3;+0:9](=[O;H0;D1;+0:10])-[CH2;D2;+0:8]-[O;H0;D2;+0:5]-[C:3]-1=[O;D1;H0:4]
60
[{"value": 60.0, "product": "CC1(OC(COC1=O)=O)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
A solution of 1 g of cyclic keto-ester (7.8 mmol), 2.7 g of metachloroperbenzoic acid (2 eq.) and 70 μl of trifluoromethanesulphonic acid (0.1 eq.) in 20 ml of dichloromethane is left under stirring at ambient temperature for 3 hours. The solvent is eliminated under vacuum, then the medium is analyzed. NMR 1H reveals t...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Tertiary halide.Tertiary halide.Tertiary halide.Peroxide.Sulfonic acid
Ester.Ester
c1ccccc1
C1COCCO1
C1COCCO1
Other
ClCCl
null
3
O=C(OO)c1cccc(Cl)c1.O=S(=O)(O)C(F)(F)F>ClCCl>CC1(C)OC(=O)COC1=O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-19d94f0f1bb1409e909c25ac1d6bf545
O=C(OO)c1cccc(Cl)c1>>CCC1(C)OC(=O)COC1=O
ClC1=CC(=CC=C1)C(=O)OO>>C(C)C1(OC(COC1=O)=O)C
Cl[c:3]1[cH:4][c:8]([C:6]([O:5][OH:7])=[O:11])[cH:2][cH:1][cH:10]1>>[CH3:1][CH2:2][C:3]1([CH3:4])[O:5][C:6](=[O:7])[CH2:8][O:9][C:10]1=[O:11]
O=C(OO)c1cccc(Cl)c1
CCC1(C)OC(=O)COC1=O
null
null
ClCCl
Miscellaneous
OtherReaction
4400727cd1198764fe8b1969daa817e812a15f25c8b234ac111afebd28f75e4d
08ae86020599855ef67800c69886dbf7915f83dafbd43cf0edc5db86fcf85ed8
O=C1COC(=O)CO1
Cl-[c;H0;D3;+0:1]1:[cH;D2;+0:2]:[cH;D2;+0:3]:[cH;D2;+0:4]:[c;H0;D3;+0:5](-[C;H0;D3;+0:6](=[O;H0;D1;+0:7])-[O;H0;D2;+0:8]-[OH;D1;+0:9]):[cH;D2;+0:10]:1>>[CH3;D1;+0:3]-[CH2;D2;+0:4]-[C;H0;D4;+0:1]1(-[CH3;D1;+0:10])-[O;H0;D2;+0:8]-[C;H0;D3;+0:6](=[O;H0;D1;+0:9])-[CH2;D2;+0:5]-[#8:11]-[C;H0;D3;+0:2]-1=[O;H0;D1;+0:7]
75
[{"value": 75.0, "product": "C(C)C1(OC(COC1=O)=O)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 0.5 g of cyclic keto-ester (3.5 mmol) and 1.21 g of metachloroperbenzoic acid (2 eq.) in 10 ml of dichloromethane is heated under reflux for 48 hours. After returning to ambient temperature, the solvent is eliminated under vacuum. NMR 1H analysis reveals the complete conversion of the ring with 5 members ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Peroxide
Ester.Ester
c1ccccc1
C1COCCO1
C1COCCO1
null
ClCCl
null
null
O=C(OO)c1cccc(Cl)c1>ClCCl>CCC1(C)OC(=O)COC1=O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-68dc893cc621422e8b91a7c12f815dad
BrBr.CC(=O)c1ccc(C(C)(C)C)cc1>>CC(C)(C)c1ccc(C(=O)CBr)cc1
CC(=O)C1=CC=C(C=C1)C(C)(C)C.BrBr.Br>>BrCC(=O)C1=CC=C(C=C1)C(C)(C)C
Br[Br:12].[CH3:1][C:2]([CH3:3])([CH3:4])[c:5]1[cH:6][cH:7][c:8]([C:9](=[O:10])[CH3:11])[cH:13][cH:14]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[c:5]1[cH:6][cH:7][c:8]([C:9](=[O:10])[CH2:11][Br:12])[cH:13][cH:14]1
BrBr.CC(=O)c1ccc(C(C)(C)C)cc1
CC(C)(C)c1ccc(C(=O)CBr)cc1
null
null
C(C)(=O)O
Functional Group Interconversion
Bromination
97ca6720945af5a02c450d33ec56e946521050f9771c27f9cfcb85f3477593f6
cb3e14519230141aa015a4cf9c960def3e60f01997e61621f62506924bfa15de
c1ccccc1
Br-[Br;H0;D1;+0:1].[CH3;D1;+0:2]-[C:3](=[O;D1;H0:4])-[c:5]>>[Br;H0;D1;+0:1]-[CH2;D2;+0:2]-[C:3](=[O;D1;H0:4])-[c:5]
null
[]
null
null
4
HOUR
A solution of 4-tert-butylacetophenone (5 g, 28.4 mmol) in acetic acid (2 mL) was carefully (the reaction was exothermic) treated with Br2 (1.46 mL, 28.5 mmol), followed by 48% aq. HBr (0.015 mL, 0.132 mmol). The reaction was stirred at room temperature for 4 hours, then was poured onto ice and was extracted with dieth...
10.6084/m9.figshare.5104873.v1
null
Ketone
Primary halide
null
null
c1ccccc1
HBr
C(C)(=O)O
null
4
BrBr.CC(=O)c1ccc(C(C)(C)C)cc1>C(C)(=O)O>CC(C)(C)c1ccc(C(=O)CBr)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5d6baec4e8404978a184d19e768cdbb6
CC(C)(C)c1ccc(C(=O)CBr)cc1.[N-]=[N+]=[N-]>>CC(C)(C)c1ccc(C(=O)CN=[N+]=[N-])cc1
[Na+].[Cl-].BrCC(=O)C1=CC=C(C=C1)C(C)(C)C.[N-]=[N+]=[N-].[Na+]>>N(=[N+]=[N-])CC(=O)C1=CC=C(C=C1)C(C)(C)C
Br[CH2:11][C:9]([c:8]1[cH:7][cH:6][c:5]([C:2]([CH3:1])([CH3:3])[CH3:4])[cH:16][cH:15]1)=[O:10].[N-:12]=[N+:13]=[N-:14]>>[CH3:1][C:2]([CH3:3])([CH3:4])[c:5]1[cH:6][cH:7][c:8]([C:9](=[O:10])[CH2:11][N:12]=[N+:13]=[N-:14])[cH:15][cH:16]1
CC(C)(C)c1ccc(C(=O)CBr)cc1.[N-]=[N+]=[N-]
CC(C)(C)c1ccc(C(=O)CN=[N+]=[N-])cc1
null
null
CC(=O)C
Heteroatom Alkylation and Arylation
OtherReaction
7fe919211b759a1428a74cb1057710661d1d522f092678548e8299963d0e0365
f47c52494d5e4df5ea8fcd9d0881525b7662fe98ccef006a42d77c12f4514758
c1ccccc1
Br-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4].[N-;H0;D1:5]=[#7;+:6]=[N;-;D1;H0:7]>>[N;-;D1;H0:7]=[#7;+:6]=[N;H0;D2;+0:5]-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]
85.3
[{"value": 85.0, "product": "N(=[N+]=[N-])CC(=O)C1=CC=C(C=C1)C(C)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 85.3, "product": "N(=[N+]=[N-])CC(=O)C1=CC=C(C=C1)C(C)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To a solution of the product of Example 1A (985 mg, 3.86 mmol) in 45 mL acetone was added NaN3 (0.505 g, 7.07 mmol), and the mixture stirred overnight at room temperature. The reaction mixture was poured into saturated NaCl solution and extracted with dichloromethane. The extracts were washed with saturated NaCl soluti...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ketone
Ketone.Azide
null
null
c1ccccc1
Br-
CC(=O)C
null
8
CC(C)(C)c1ccc(C(=O)CBr)cc1.[N-]=[N+]=[N-]>CC(=O)C>CC(C)(C)c1ccc(C(=O)CN=[N+]=[N-])cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3cc7c50802ec48e0a693d4bfa31dc99d
CCOc1ccc2cccc(NC(=O)OC(C)(C)C)c2c1>>CCOc1ccc2cccc(N)c2c1
C(C)OC1=CC=C2C=CC=C(C2=C1)NC(OC(C)(C)C)=O.Cl>>C(C)OC1=CC=C2C=CC=C(C2=C1)N
CC(C)(C)OC(=O)[NH:12][c:11]1[cH:10][cH:9][cH:8][c:7]2[cH:6][cH:5][c:4]([O:3][CH2:2][CH3:1])[cH:14][c:13]21>>[CH3:1][CH2:2][O:3][c:4]1[cH:5][cH:6][c:7]2[cH:8][cH:9][cH:10][c:11]([NH2:12])[c:13]2[cH:14]1
CCOc1ccc2cccc(NC(=O)OC(C)(C)C)c2c1
CCOc1ccc2cccc(N)c2c1
null
null
O1CCOCC1.C(C)OCC
Reduction
Hydrogenolysis of amides/imides/carbamates
3c33dd2a2d355ee5ba0287367e209aa147a39aa00607f0c95fb2bf1ade45d014
c5b5dffe7dd8beebdc1baa8b5b05300a9f7079e65dcfd42ade6f8a77ff09537d
c1ccc2ccccc2c1
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
52
[{"value": 52.0, "product": "C(C)OC1=CC=C2C=CC=C(C2=C1)N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 51.7, "product": "C(C)OC1=CC=C2C=CC=C(C2=C1)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3.5
HOUR
To a solution of the product of Example 1C (14.47 g, 50.4 mmol) in dioxane (30 mL) at 0° C. was added 4N HCl in dioxane (60 mL, 240 mmol). The reaction mixture was stirred at room temperature for 3.5 hours, diluted with 3 volumes of diethyl ether. The resulting dark brown precipitate was collected by filtration. It was...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Primary amine
null
null
c1ccc2ccccc2c1
HO-
O1CCOCC1.C(C)OCC
null
3.5
CCOc1ccc2cccc(NC(=O)OC(C)(C)C)c2c1>O1CCOCC1.C(C)OCC>CCOc1ccc2cccc(N)c2c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-11a81ffe826b44e89ced61ff8a22bd07
CCOc1ccc2cccc(N)c2c1>>CCOC1=CCc2cccc(N)c2C1
[Li].C(C)OC1=CC=C2C=CC=C(C2=C1)N.C(C)(C)(C)O.N>>C(C)OC1=CCC=2C=CC=C(C2C1)N
[CH3:1][CH2:2][O:3][c:4]1[cH:5][cH:6][c:7]2[cH:8][cH:9][cH:10][c:11]([NH2:12])[c:13]2[cH:14]1>>[CH3:1][CH2:2][O:3][C:4]1=[CH:5][CH2:6][c:7]2[cH:8][cH:9][cH:10][c:11]([NH2:12])[c:13]2[CH2:14]1
CCOc1ccc2cccc(N)c2c1
CCOC1=CCc2cccc(N)c2C1
null
null
O1CCCC1
Miscellaneous
OtherReaction
47cfb58d0c1d97c9a88a3f7fa92108ac5ffdcba9a9b8195e99d4dfecb292a8df
bced64702950df7cf56df22d8c2487b007734fece951727fd2c8a1c63fbcf6cc
C1=CCc2ccccc2C1
[C:1]-[#8:2]-[c;H0;D3;+0:3]1:[cH;D2;+0:4]:[c:5](:[c:6]):[c:7](:[c:8]):[cH;D2;+0:9]:[cH;D2;+0:10]:1>>[C:1]-[#8:2]-[C;H0;D3;+0:3]1=[CH;D2;+0:10]-[CH2;D2;+0:9]-[c:7](:[c:8]):[c:5](:[c:6])-[CH2;D2;+0:4]-1
55
[{"value": 55.0, "product": "C(C)OC1=CCC=2C=CC=C(C2C1)N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 54.8, "product": "C(C)OC1=CCC=2C=CC=C(C2C1)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-78
CELSIUS
1
HOUR
The product of Example 1D (1.8 g, 9.63 mmol) and tert-butanol (2.13 g, 28.8 mmol) were dissolved in tetrahydrofuran (20 mL) in a 3-neck 1000 mL round-bottom flask, and the solution was cooled to −78° C. Ammonia (˜35 mL) was condensed into the flask, then lithium metal was added (wire, 225 mg, 32.4 mmol) in portions ove...
10.6084/m9.figshare.5104873.v1
null
Ether
Ether
c1ccc2ccccc2c1
C1=CCc2ccccc2C1
C1=CCc2ccccc2C1
null
O1CCCC1
-78
1
CCOc1ccc2cccc(N)c2c1>O1CCCC1>CCOC1=CCc2cccc(N)c2C1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5ba29fd898794ebf8e3230da2c8c99f0
CCOC1=CCc2cccc(N)c2C1.S=C(Oc1ccccn1)Oc1ccccn1>>CCOC1=CCc2cccc(N=C=S)c2C1
C(C)OC1=CCC=2C=CC=C(C2C1)N.C(OC1=NC=CC=C1)(OC1=NC=CC=C1)=S>>C(C)OC=1CC2=C(C=CC=C2CC1)N=C=S
[CH3:1][CH2:2][O:3][C:4]1=[CH:5][CH2:6][c:7]2[cH:8][cH:9][cH:10][c:11]([NH2:12])[c:15]2[CH2:16]1.c1ccc(O[C:13](Oc2ccccn2)=[S:14])nc1>>[CH3:1][CH2:2][O:3][C:4]1=[CH:5][CH2:6][c:7]2[cH:8][cH:9][cH:10][c:11]([N:12]=[C:13]=[S:14])[c:15]2[CH2:16]1
CCOC1=CCc2cccc(N)c2C1.S=C(Oc1ccccn1)Oc1ccccn1
CCOC1=CCc2cccc(N=C=S)c2C1
null
null
ClCCl
Heteroatom Alkylation and Arylation
OtherReaction
9a80968abe70879a9369740fc6263b884e7d64cc7f090788997500a3069df240
0bc85fa9e96d94388afe13d389361cafe3d77a7182964e359eefb70b6e8160bc
C1=CCc2ccccc2C1
[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4].[S;D1;H0:5]=[C;H0;D3;+0:6](-O-c1:c:c:c:c:n:1)-O-c1:c:c:c:c:n:1>>[S;D1;H0:5]=[C;H0;D2;+0:6]=[N;H0;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
18
HOUR
A solution of the product of Example 1E (200 mg, 1.06 mmol) in dichloromethane (2.5 mL) was added to a solution of O,O-dipyridin-2-yl thiocarbonate (246 mg, 1.06 mmol) in dichloromethane (5 mL) at room temperature. After stirring at room temperature for 18 hours, the mixture was concentrated, then filtered through sili...
10.6084/m9.figshare.5104873.v1
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Ether.Ether.Primary amine.Thiocarbonyl
Isothiocyanate
c1ccncc1.c1ccncc1
null
C1=CCc2ccccc2C1
HO-
ClCCl
null
18
CCOC1=CCc2cccc(N)c2C1.S=C(Oc1ccccn1)Oc1ccccn1>ClCCl>CCOC1=CCc2cccc(N=C=S)c2C1