dataset_id
large_stringclasses
414 values
reaction_id
large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
reactant_smiles
large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-bff2a076ce534e20a3ef04c541e07fc6
N.O=C(NS(=O)(=O)c1ccc(Cl)c([N+](=O)[O-])c1)c1ccc(-c2ccc(F)cc2)cc1>>Nc1ccc(S(=O)(=O)NC(=O)c2ccc(-c3ccc(F)cc3)cc2)cc1[N+](=O)[O-]
ClC1=C(C=C(C=C1)S(=O)(=O)NC(=O)C1=CC=C(C=C1)C1=CC=C(C=C1)F)[N+](=O)[O-].N>>NC1=C(C=C(C=C1)S(=O)(=O)NC(=O)C1=CC=C(C=C1)C1=CC=C(C=C1)F)[N+](=O)[O-]
[NH3:1].Cl[c:2]1[cH:3][cH:4][c:5]([S:6](=[O:7])(=[O:8])[NH:9][C:10](=[O:11])[c:12]2[cH:13][cH:14][c:15](-[c:16]3[cH:17][cH:18][c:19]([F:20])[cH:21][cH:22]3)[cH:23][cH:24]2)[cH:25][c:26]1[N+:27](=[O:28])[O-:29]>>[NH2:1][c:2]1[cH:3][cH:4][c:5]([S:6](=[O:7])(=[O:8])[NH:9][C:10](=[O:11])[c:12]2[cH:13][cH:14][c:15](-[c:16]3...
N.O=C(NS(=O)(=O)c1ccc(Cl)c([N+](=O)[O-])c1)c1ccc(-c2ccc(F)cc2)cc1
Nc1ccc(S(=O)(=O)NC(=O)c2ccc(-c3ccc(F)cc3)cc2)cc1[N+](=O)[O-]
null
null
CO.C(C)(=O)OCC
Heteroatom Alkylation and Arylation
OtherReaction
5cea7b75c7f95cc50fd74029efa1cddce51f01200160afa4aaecfa45e52a1621
c5668f64a1395fa45312378ed819baaeafc354cdb673b20226ea2853ed14db5d
O=C(NS(=O)(=O)c1ccccc1)c1ccc(-c2ccccc2)cc1
Cl-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[#7;+:5]):[c:6].[NH3;D0;+0:7]>>[#7;+:5]-[c:4](:[c:6]):[c;H0;D3;+0:1](-[NH2;D1;+0:7]):[c:2]:[c:3]
null
[]
0
CELSIUS
null
null
A solution of Example 1D (1.0 g) in methanol (10 mL) and concentrated aqueous ammonia (3 mL) was heated in a sealed pressure tube to 60° C. for 16 hours, cooled to 0° C., diluted with ethyl acetate (100 mL), washed with water (30 mL) and brine (10 mL), dried (MgSO4), filtered, and concentrated to provide the desired pr...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
Primary amine
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1.c1ccccc1
HCl
CO.C(C)(=O)OCC
0
null
N.O=C(NS(=O)(=O)c1ccc(Cl)c([N+](=O)[O-])c1)c1ccc(-c2ccc(F)cc2)cc1>CO.C(C)(=O)OCC>Nc1ccc(S(=O)(=O)NC(=O)c2ccc(-c3ccc(F)cc3)cc2)cc1[N+](=O)[O-]
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8d3b28bfd0764d53ae5724cb43a3f362
Nc1ccc(S(=O)(=O)NC(=O)c2ccc(-c3ccc(F)cc3)cc2)cc1[N+](=O)[O-].O=C(Cl)C12CC3CC(CC(C3)C1)C2>>O=C(NS(=O)(=O)c1ccc(NC(=O)C23CC4CC(CC(C4)C2)C3)c([N+](=O)[O-])c1)c1ccc(-c2ccc(F)cc2)cc1
C12(CC3CC(CC(C1)C3)C2)C(=O)Cl.NC1=C(C=C(C=C1)S(=O)(=O)NC(=O)C1=CC=C(C=C1)C1=CC=C(C=C1)F)[N+](=O)[O-].[H-].[Na+].Cl>>FC1=CC=C(C=C1)C1=CC=C(C=C1)C(=O)NS(=O)(=O)C1=CC(=C(C=C1)NC(=O)C12CC3CC(CC(C1)C3)C2)[N+](=O)[O-]
[O:1]=[C:2]([NH:3][S:4](=[O:5])(=[O:6])[c:7]1[cH:8][cH:9][c:10]([NH2:11])[c:24]([N+:25](=[O:26])[O-:27])[cH:28]1)[c:29]1[cH:30][cH:31][c:32](-[c:33]2[cH:34][cH:35][c:36]([F:37])[cH:38][cH:39]2)[cH:40][cH:41]1.Cl[C:12](=[O:13])[C:14]12[CH2:15][CH:16]3[CH2:17][CH:18]([CH2:19][CH:20]([CH2:21]3)[CH2:22]1)[CH2:23]2>>[O:1]=[...
Nc1ccc(S(=O)(=O)NC(=O)c2ccc(-c3ccc(F)cc3)cc2)cc1[N+](=O)[O-].O=C(Cl)C12CC3CC(CC(C3)C1)C2
O=C(NS(=O)(=O)c1ccc(NC(=O)C23CC4CC(CC(C4)C2)C3)c([N+](=O)[O-])c1)c1ccc(-c2ccc(F)cc2)cc1
null
null
O1CCOCC1
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
O=C(NS(=O)(=O)c1ccc(NC(=O)C23CC4CC(CC(C4)C2)C3)cc1)c1ccc(-c2ccccc2)cc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])(-[C:5])-[C:6].[NH2;D1;+0:7]-[c:8](:[c:9]):[c:10]>>[C:4]-[C:3](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:7]-[c:8](:[c:9]):[c:10])(-[C:5])-[C:6]
null
[]
null
null
30
MINUTE
A solution of Example 380A (101 mg, 0.25 mmol) in TBF (3 mL) was treated with 60% sodium hydride in oil (40 mg, 1.0 mmol), stirred for 30 minutes, treated with 1-adamantanecarbonyl chloride (60 mg, 0.30 mmol), stirred for 30 minutes, adjusted to pH<7 with 4M HCl in dioxane (0.5 mL), filtered, and concentrated. The conc...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccccc1.c1ccccc1.C1C2CC3CC1CC(C2)C3
HCl
O1CCOCC1
null
0.5
Nc1ccc(S(=O)(=O)NC(=O)c2ccc(-c3ccc(F)cc3)cc2)cc1[N+](=O)[O-].O=C(Cl)C12CC3CC(CC(C3)C1)C2>O1CCOCC1>O=C(NS(=O)(=O)c1ccc(NC(=O)C23CC4CC(CC(C4)C2)C3)c([N+](=O)[O-])c1)c1ccc(-c2ccc(F)cc2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5097bcb7a27844ffac144da89958c1e3
COC(=O)c1ccc(B(O)O)cc1.Cc1c(C#N)sc2ccc(Cl)cc12>>COC(=O)c1ccc(-c2ccc3sc(C#N)c(C)c3c2)cc1
ClC=1C=CC2=C(C(=C(S2)C#N)C)C1.COC(=O)C1=CC=C(C=C1)B(O)O.C(C)(C)(C)P(C1=C(C=CC=C1)C1=CC=CC=C1)C(C)(C)C.[F-].[K+]>>C(#N)C=1SC2=C(C1C)C=C(C=C2)C2=CC=C(C(=O)OC)C=C2
OB(O)[c:8]1[cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:22][cH:21]1.Cl[c:9]1[cH:10][cH:11][c:12]2[s:13][c:14]([C:15]#[N:16])[c:17]([CH3:18])[c:19]2[cH:20]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8](-[c:9]2[cH:10][cH:11][c:12]3[s:13][c:14]([C:15]#[N:16])[c:17]([CH3:18])[c:19]3[cH:20]2)[cH:21][cH:22]1
COC(=O)c1ccc(B(O)O)cc1.Cc1c(C#N)sc2ccc(Cl)cc12
COC(=O)c1ccc(-c2ccc3sc(C#N)c(C)c3c2)cc1
null
CC(=O)[O-].CC(=O)[O-].[Pd+2]
C1CCOC1
C-C Coupling
Suzuki coupling with boronic acids
a1259a94b31ac9f1988cb839e0910c5b2437b7522341904299ff46277eacea87
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc3sccc3c2)cc1
Cl-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](:[#16;a:5]):[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[#16;a:5]:[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]):[c:7]:[c:6]:1
null
[]
null
null
null
null
A mixture of Example 401A (557 mg, 2.68 mmol), (4-methoxycarbonylphenyl)-boronic acid (675 mg, 3.75 mmol), Pd(OAc)2 (36 mg, 0.16 mmol), 2-(di-tert-butylphosphino)biphenyl (63 mg, 0.21 mmol), and KF (467 mg, 8.04 mmol) in THF (10mL) was heated to 60° C. for 16 hours and concentrated The concentrate was purified by flash...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccc2sccc2c1
c1ccccc1.c1ccc2sccc2c1
c1ccccc1.c1ccc2sccc2c1
HCl.B
CC(=O)[O-].CC(=O)[O-].[Pd+2].C1CCOC1
null
null
COC(=O)c1ccc(B(O)O)cc1.Cc1c(C#N)sc2ccc(Cl)cc12>CC(=O)[O-].CC(=O)[O-].[Pd+2].C1CCOC1>COC(=O)c1ccc(-c2ccc3sc(C#N)c(C)c3c2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1ce22d6cab7d4438bd93a5a0416d7bf2
CI.COC(=O)c1ccc(-c2ccc(CO)cc2OC)cc1>>COCc1ccc(-c2ccc(C(=O)OC)cc2)c(OC)c1
OCC1=CC(=C(C=C1)C1=CC=C(C=C1)C(=O)OC)OC.[H-].[Na+].CI.Cl>>COC1=C(C=CC(=C1)COC)C1=CC=C(C=C1)C(=O)OC
I[CH3:1].[OH:2][CH2:3][c:4]1[cH:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][c:11]([C:12](=[O:13])[O:14][CH3:15])[cH:16][cH:17]2)[c:18]([O:19][CH3:20])[cH:21]1>>[CH3:1][O:2][CH2:3][c:4]1[cH:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][c:11]([C:12](=[O:13])[O:14][CH3:15])[cH:16][cH:17]2)[c:18]([O:19][CH3:20])[cH:21]1
CI.COC(=O)c1ccc(-c2ccc(CO)cc2OC)cc1
COCc1ccc(-c2ccc(C(=O)OC)cc2)c(OC)c1
null
null
O1CCOCC1.C1CCOC1
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
31b37b19ff6de58cf584e89bae19f862b01d058b473835fea10bbd4c0a53fd14
f3e76c16e7df5a83f618c93f8745117d548e410efce45e89753f2c180a9b20f8
c1ccc(-c2ccccc2)cc1
I-[CH3;D1;+0:1].[OH;D1;+0:2]-[C:3]-[c:4]>>[CH3;D1;+0:1]-[O;H0;D2;+0:2]-[C:3]-[c:4]
null
[]
null
null
30
MINUTE
A solution of Example 417A (142 mg, 0.5 mmol) in THF (3 mL) at room temperature was treated with 60% sodium hydride in oil (40 mg, 1.0 mmol) and methyl iodide (0.30 mmol), stirred for 30 minutes, adjusted to pH<7 with 4M HCl in dioxane (0.5 mL), filtered, and concentrated. The concentrate was purified by flash column c...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Ether
null
null
c1ccccc1.c1ccccc1
HI
O1CCOCC1.C1CCOC1
null
0.5
CI.COC(=O)c1ccc(-c2ccc(CO)cc2OC)cc1>O1CCOCC1.C1CCOC1>COCc1ccc(-c2ccc(C(=O)OC)cc2)c(OC)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7b00705408e44469941c490f5be2f99e
COC(=O)c1ccc(C2=CCC3(CC2)OCCO3)cc1>>COC(=O)c1ccc(C2=CCC(=O)CC2)cc1
O1CCOC12CC=C(CC2)C2=CC=C(C(=O)OC)C=C2.C1(=CC=C(C=C1)S(=O)(=O)O)C>>O=C1CC=C(CC1)C1=CC=C(C(=O)OC)C=C1
C1C[O:13][C:12]2(O1)[CH2:11][CH:10]=[C:9]([c:8]1[cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:17][cH:16]1)[CH2:15][CH2:14]2>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([C:9]2=[CH:10][CH2:11][C:12](=[O:13])[CH2:14][CH2:15]2)[cH:16][cH:17]1
COC(=O)c1ccc(C2=CCC3(CC2)OCCO3)cc1
COC(=O)c1ccc(C2=CCC(=O)CC2)cc1
null
null
CC(=O)C
Miscellaneous
Ketal hydrolysis to ketone
28bfec55e245adc574605e1d0e9aea134d32b54ad000fbfecce09d058b7f56f3
547697208447432e865290cf95eed8e4fcddc12f59856b7ddbf24dc1accb1210
O=C1CC=C(c2ccccc2)CC1
[c:1]-[C:2]1=[C:3]-[C:4]-[C;H0;D4;+0:5]2(-O-C-C-[O;H0;D2;+0:6]-2)-[C:7]-[C:8]-1>>[O;H0;D1;+0:6]=[C;H0;D3;+0:5]1-[C:4]-[C:3]=[C:2](-[c:1])-[C:8]-[C:7]-1
null
[]
null
null
null
null
A solution of Example 420B (2.2 g) and p-toluenesulfonic acid (100 mg) in acetone (10 mL) was heated to reflux for 10 hours, filtered through a pad of silica gel (20 g), and concentrated to provide the desired product. Conditions: See reaction.notes.procedure_details. Workup: to reflux for 10 hours; filtered through a ...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether
Ketone
C1=CCC2(CC1)OCCO2
C1=CCCCC1
c1ccccc1.C1=CCCCC1
HO-
CC(=O)C
null
null
COC(=O)c1ccc(C2=CCC3(CC2)OCCO3)cc1>CC(=O)C>COC(=O)c1ccc(C2=CCC(=O)CC2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-21e914593c374e0cac9a20bb9660e89a
COC(=O)c1ccc(C2=CCC(=O)CC2)cc1>>COC(=O)c1ccc(C2=CCC(C)(O)CC2)cc1
O=C1CC=C(CC1)C1=CC=C(C(=O)OC)C=C1.C[Li].[Cl-].[Ce+3].[Cl-].[Cl-].[Cl-].[Li+]>>OC1(CC=C(CC1)C1=CC=C(C(=O)OC)C=C1)C
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([C:9]2=[CH:10][CH2:11][C:12](=[O:14])[CH2:15][CH2:16]2)[cH:17][cH:18]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([C:9]2=[CH:10][CH2:11][C:12]([CH3:13])([OH:14])[CH2:15][CH2:16]2)[cH:17][cH:18]1
COC(=O)c1ccc(C2=CCC(=O)CC2)cc1
COC(=O)c1ccc(C2=CCC(C)(O)CC2)cc1
null
null
C(C)(=O)OCC.C(C)OCC.C1CCOC1
Miscellaneous
OtherReaction
82f307c2771f24472352179bfdcbd50ca1b6a8d7cf7b2748b565724a523407a8
8811b4d793f7cfa9f0f1f47a008648edabb54f371f76dfa680dd5b2e1564c6c5
C1=C(c2ccccc2)CCCC1
[O;H0;D1;+0:1]=[C;H0;D3;+0:2]1-[C:3]-[C:4]=[C:5](-[c:6])-[C:7]-[C:8]-1>>[C;D1;H3:9]-[C;H0;D4;+0:2]1(-[OH;D1;+0:1])-[C:3]-[C:4]=[C:5](-[c:6])-[C:7]-[C:8]-1
null
[]
null
null
null
null
A suspension of anhydrous cerium(III) chloride (2.71 g, 11 mmol) in THF (10 mL) at −78° C. was slowly treated with 1.5M methyllithium complexed with lithium chloride in diethyl ether (6.7 mL), warmed to room temperature over 2 hours, and added to a solution of Example 420C (1.15 g, 5.0mmol) in THF (10 mL) at −78° C. Th...
10.6084/m9.figshare.5104873.v1
null
Ketone
Tertiary alcohol
C1=CCCCC1
C1=CCCCC1
c1ccccc1.C1=CCCCC1
Other
C(C)(=O)OCC.C(C)OCC.C1CCOC1
null
null
COC(=O)c1ccc(C2=CCC(=O)CC2)cc1>C(C)(=O)OCC.C(C)OCC.C1CCOC1>COC(=O)c1ccc(C2=CCC(C)(O)CC2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b476166e14714a7e91095eac307ce4e4
COC(=O)[C@H](CSc1ccccc1)Nc1ccc(S(N)(=O)=O)cc1[N+](=O)[O-]>>NS(=O)(=O)c1ccc(NC(CO)CSc2ccccc2)c([N+](=O)[O-])c1
NS(=O)(=O)C1=CC(=C(C=C1)N[C@@H](CSC1=CC=CC=C1)C(=O)OC)[N+](=O)[O-].[BH4-].[Li+]>>OCC(CSC1=CC=CC=C1)NC1=C(C=C(C=C1)S(=O)(=O)N)[N+](=O)[O-]
CO[C:11]([C@@H:10]([NH:9][c:8]1[cH:7][cH:6][c:5]([S:2]([NH2:1])(=[O:3])=[O:4])[cH:25][c:21]1[N+:22](=[O:23])[O-:24])[CH2:13][S:14][c:15]1[cH:16][cH:17][cH:18][cH:19][cH:20]1)=[O:12]>>[NH2:1][S:2](=[O:3])(=[O:4])[c:5]1[cH:6][cH:7][c:8]([NH:9][CH:10]([CH2:11][OH:12])[CH2:13][S:14][c:15]2[cH:16][cH:17][cH:18][cH:19][cH:20...
COC(=O)[C@H](CSc1ccccc1)Nc1ccc(S(N)(=O)=O)cc1[N+](=O)[O-]
NS(=O)(=O)c1ccc(NC(CO)CSc2ccccc2)c([N+](=O)[O-])c1
null
null
CO.C(C)(=O)OCC.C1CCOC1
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
c1ccc(NCCSc2ccccc2)cc1
C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[C@@H;D3;+0:3](-[#7:4]-[c:5])-[C:6]-[#16:7]>>[#16:7]-[C:6]-[CH;D3;+0:3](-[#7:4]-[c:5])-[CH2;D2;+0:1]-[OH;D1;+0:2]
null
[]
null
null
3
HOUR
A solution of Example 434A (1.42 g, 3.45 mmol) in THF (10 mL) and methanol (1 mL) at room temperature was slowly treated with lithium borohydride (100 mg), stirred for 3 hours, as diluted with ethyl acetate (100 mL), washed with water (45 mL) and brine (10 mL), dried (MgSO4), filtered, and concentrated to provide the d...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
c1ccccc1.c1ccccc1
Other
CO.C(C)(=O)OCC.C1CCOC1
null
3
COC(=O)[C@H](CSc1ccccc1)Nc1ccc(S(N)(=O)=O)cc1[N+](=O)[O-]>CO.C(C)(=O)OCC.C1CCOC1>NS(=O)(=O)c1ccc(NC(CO)CSc2ccccc2)c([N+](=O)[O-])c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-87ebc5f3cd504bc8920c2b08ab1bf8b6
NS(=O)(=O)c1ccc(NC(CO)CSc2ccccc2)c([N+](=O)[O-])c1.[N-]=[N+]=[N-]>>[N-]=[N+]=NCC(CSc1ccccc1)Nc1ccc(S(N)(=O)=O)cc1[N+](=O)[O-]
OCC(CSC1=CC=CC=C1)NC1=C(C=C(C=C1)S(=O)(=O)N)[N+](=O)[O-].C(C)(C)N(C(C)C)CC.CS(=O)(=O)Cl.[N-]=[N+]=[N-].[Na+]>>N(=[N+]=[N-])CC(CSC1=CC=CC=C1)NC1=C(C=C(C=C1)S(=O)(=O)N)[N+](=O)[O-]
O[CH2:4][CH:5]([CH2:6][S:7][c:8]1[cH:9][cH:10][cH:11][cH:12][cH:13]1)[NH:14][c:15]1[cH:16][cH:17][c:18]([S:19]([NH2:20])(=[O:21])=[O:22])[cH:23][c:24]1[N+:25](=[O:26])[O-:27].[N-:1]=[N+:2]=[N-:3]>>[N-:1]=[N+:2]=[N:3][CH2:4][CH:5]([CH2:6][S:7][c:8]1[cH:9][cH:10][cH:11][cH:12][cH:13]1)[NH:14][c:15]1[cH:16][cH:17][c:18]([...
NS(=O)(=O)c1ccc(NC(CO)CSc2ccccc2)c([N+](=O)[O-])c1.[N-]=[N+]=[N-]
[N-]=[N+]=NCC(CSc1ccccc1)Nc1ccc(S(N)(=O)=O)cc1[N+](=O)[O-]
null
[I-].C(CCC)[N+](CCCC)(CCCC)CCCC
ClCCl.CN(C)C=O.C(C)(=O)OCC
Functional Group Addition
OtherReaction
f9a80609465600bf0decaa33fd5de5feaf004c5d380786fc66eb0efb9e034bbe
9decb3955913485691906a27715d754335868709c17a134aab1e5b87ceb0a1d6
c1ccc(NCCSc2ccccc2)cc1
O-[CH2;D2;+0:1]-[C:2](-[#7:3])-[C:4].[N-;H0;D1:5]=[#7;+:6]=[N;-;D1;H0:7]>>[#7:3]-[C:2](-[C:4])-[CH2;D2;+0:1]-[N;H0;D2;+0:5]=[#7;+:6]=[N;-;D1;H0:7]
null
[]
50
CELSIUS
1
HOUR
A solution of Example 434B (1.01 g, 2.6 mmol) and N,N-diisopropylethylamine (0.70 mL, 4.0 mmol) in dichloromethane (5 mL) and DMF (5 mL) at room temperature was treated with methanesulfonyl chloride (0.22 mL, 2.90 mmol), stirred for 1 hour, and concentrated to remove the dichloromethane. The resulting DMF solution was ...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Azide
null
null
c1ccccc1.c1ccccc1
HO-
[I-].C(CCC)[N+](CCCC)(CCCC)CCCC.ClCCl.CN(C)C=O.C(C)(=O)OCC
50
1
NS(=O)(=O)c1ccc(NC(CO)CSc2ccccc2)c([N+](=O)[O-])c1.[N-]=[N+]=[N-]>[I-].C(CCC)[N+](CCCC)(CCCC)CCCC.ClCCl.CN(C)C=O.C(C)(=O)OCC>[N-]=[N+]=NCC(CSc1ccccc1)Nc1ccc(S(N)(=O)=O)cc1[N+](=O)[O-]
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-333c17c03f8044eb9956ea3aae74859d
BrCc1ccccc1.COC(=O)C(CO)NC(=O)OC(C)(C)C>>COC(=O)[C@H](COCc1ccccc1)NC(=O)OC(C)(C)C
N(C(CO)C(=O)OC)C(=O)OC(C)(C)C.C(C1=CC=CC=C1)Br>>C(C1=CC=CC=C1)OC[C@H](NC(=O)OC(C)(C)C)C(=O)OC
Br[CH2:8][c:9]1[cH:10][cH:11][cH:12][cH:13][cH:14]1.[CH3:1][O:2][C:3](=[O:4])[CH:5]([CH2:6][OH:7])[NH:15][C:16](=[O:17])[O:18][C:19]([CH3:20])([CH3:21])[CH3:22]>>[CH3:1][O:2][C:3](=[O:4])[C@H:5]([CH2:6][O:7][CH2:8][c:9]1[cH:10][cH:11][cH:12][cH:13][cH:14]1)[NH:15][C:16](=[O:17])[O:18][C:19]([CH3:20])([CH3:21])[CH3:22]
BrCc1ccccc1.COC(=O)C(CO)NC(=O)OC(C)(C)C
COC(=O)[C@H](COCc1ccccc1)NC(=O)OC(C)(C)C
null
[Ag]=O
ClCCl
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
dd3f9c60e1f90d961a7c01d970ae213561355ee1451f276a3b04696e4b6fae5c
46a6e883cf919b4006e69abfdfd883f458f55c08b3200960c6a5b57c4139fbca
c1ccccc1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[#8:5]-[C:6](=[O;D1;H0:7])-[C:8]-[C:9]-[OH;D1;+0:10]>>[#8:5]-[C:6](=[O;D1;H0:7])-[C:8]-[C:9]-[O;H0;D2;+0:10]-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
2
DAY
A mixture of BOC-DL-Ser-OMe (434 mg, 2.0 mmol), benzyl bromide (513 mg, 3.0 mmol), and silver oxide (695 mg, 3.0 mmol) in dichloromethane (10 mL) at room temperature was stirred for 2 days, filtered, and concentrated. The concentrate was purified by flash column chromatography on silica gel with 20% ethyl acetate/hexan...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary alcohol
Ether
null
null
c1ccccc1
HBr
[Ag]=O.ClCCl
null
48
BrCc1ccccc1.COC(=O)C(CO)NC(=O)OC(C)(C)C>[Ag]=O.ClCCl>COC(=O)[C@H](COCc1ccccc1)NC(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-cb05855d74514f13ba559f79a9468752
COC(=O)c1ccc(-c2ccc(C=O)cc2OC)cc1.C[Si](C)(C)[N-][Si](C)(C)C>>C=Cc1ccc(-c2ccc(C(=O)OC)cc2)c(OC)c1
C(=O)C1=CC(=C(C=C1)C1=CC=C(C=C1)C(=O)OC)OC.C[Si](C)(C)[N-][Si](C)(C)C.[Li+]>>COC1=C(C=CC(=C1)C=C)C1=CC=C(C=C1)C(=O)OC
O=[CH:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([C:11](=[O:12])[O:13][CH3:14])[cH:15][cH:16]2)[c:17]([O:18][CH3:19])[cH:20]1.C[Si](C)(C)[N-][Si](C)(C)[CH3:1]>>[CH2:1]=[CH:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([C:11](=[O:12])[O:13][CH3:14])[cH:15][cH:16]2)[c:17]([O:18][CH3:19])[cH:20]1
COC(=O)c1ccc(-c2ccc(C=O)cc2OC)cc1.C[Si](C)(C)[N-][Si](C)(C)C
C=Cc1ccc(-c2ccc(C(=O)OC)cc2)c(OC)c1
null
[Br-].C[P+](C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1
C1CCOC1
C-C Coupling
OtherReaction
65846b40393caf810f4a2d80980311afbe6a487d5b2731f135215f55a25e4832
37f02ff997533d11a1e569347ef78cf65235ab0024b34a145afdaafd2d3d15ac
c1ccc(-c2ccccc2)cc1
C-[Si](-C)(-C)-[N-]-[Si](-C)(-C)-[CH3;D1;+0:1].O=[CH;D2;+0:2]-[c:3](:[c:4]):[c:5]>>[CH2;D1;+0:1]=[CH;D2;+0:2]-[c:3](:[c:4]):[c:5]
null
[]
null
null
30
MINUTE
A suspension of methyltriphenylphosphonium bromide (785 mg, 2.2 mmoL) in THF (5 mL) was treated with 1M lithium bis(trimethylsilyl)amide in THF (2.2 mL), stirred for 30 minutes, treated with a solution of Example 122I (540 mg, 2.0 mmol) in TB (2 mL), stirred for 1 hour, and filtered through a pad of silica gel (20 g). ...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Silyl protective group.Silyl protective group
Vinyl
null
null
c1ccccc1.c1ccccc1
HO-
[Br-].C[P+](C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1.C1CCOC1
null
0.5
COC(=O)c1ccc(-c2ccc(C=O)cc2OC)cc1.C[Si](C)(C)[N-][Si](C)(C)C>[Br-].C[P+](C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1.C1CCOC1>C=Cc1ccc(-c2ccc(C(=O)OC)cc2)c(OC)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-68ccfbd23c22430fbe233f1b14b1e167
C=Cc1ccc(-c2ccc(C(=O)OC)cc2)c(OC)c1.OO>>COC(=O)c1ccc(-c2ccc(CCO)cc2OC)cc1
COC1=C(C=CC(=C1)C=C)C1=CC=C(C=C1)C(=O)OC.B.C([O-])([O-])=O.[Na+].[Na+].OO>>OCCC1=CC(=C(C=C1)C1=CC=C(C=C1)C(=O)OC)OC
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8](-[c:9]2[cH:10][cH:11][c:12]([CH:13]=[CH2:14])[cH:16][c:17]2[O:18][CH3:19])[cH:20][cH:21]1.O[OH:15]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8](-[c:9]2[cH:10][cH:11][c:12]([CH2:13][CH2:14][OH:15])[cH:16][c:17]2[O:18][CH3:19])[cH:20][cH:21]1
C=Cc1ccc(-c2ccc(C(=O)OC)cc2)c(OC)c1.OO
COC(=O)c1ccc(-c2ccc(CCO)cc2OC)cc1
null
null
C(C)(=O)OCC.C1CCOC1
Heteroatom Alkylation and Arylation
OtherReaction
6aaa6688cc4965019d9400c93c20e1d817a445418a6601722f66df7d420427e9
4ceb30033bcfd57c382fe05e353b68e7f657859dbacaaa785451a244b2657476
c1ccc(-c2ccccc2)cc1
O-[OH;D1;+0:1].[CH2;D1;+0:2]=[CH;D2;+0:3]-[c:4](:[c:5]):[c:6]>>[OH;D1;+0:1]-[CH2;D2;+0:2]-[CH2;D2;+0:3]-[c:4](:[c:5]):[c:6]
null
[]
60
CELSIUS
null
null
A solution of Example 445A (228 mg) and 1M borane in THF (1.2 mL) in THF (2 mL) at room temperature was stirred for 5 hours, and treated sequentially with 2M sodium carbonate (1 mL) and 33% hydrogen peroxide (1 mL). The mixture was heated to 60° C. for 1 hour, diluted with ethyl acetate (100 mL), washed with water (45 ...
10.6084/m9.figshare.5104873.v1
null
Peroxide.Vinyl
Primary alcohol
null
null
c1ccccc1.c1ccccc1
Other
C(C)(=O)OCC.C1CCOC1
60
null
C=Cc1ccc(-c2ccc(C(=O)OC)cc2)c(OC)c1.OO>C(C)(=O)OCC.C1CCOC1>COC(=O)c1ccc(-c2ccc(CCO)cc2OC)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a6219332344d417b859e800de0151d39
COC(=O)c1ccc(-c2ccc(CCCO[Si](C)(C)C(C)(C)C)cc2OC)cc1>>COc1cc(CCCO[Si](C)(C)C(C)(C)C)ccc1-c1ccc(C(=O)O)cc1
[Si](C)(C)(C(C)(C)C)OCCCC1=CC(=C(C=C1)C1=CC=C(C=C1)C(=O)OC)OC.[Li+].[OH-]>>[Si](C)(C)(C(C)(C)C)OCCCC1=CC(=C(C=C1)C1=CC=C(C=C1)C(=O)O)OC
C[O:26][C:24]([c:23]1[cH:22][cH:21][c:20](-[c:19]2[c:3]([O:2][CH3:1])[cH:4][c:5]([CH2:6][CH2:7][CH2:8][O:9][Si:10]([CH3:11])([CH3:12])[C:13]([CH3:14])([CH3:15])[CH3:16])[cH:17][cH:18]2)[cH:28][cH:27]1)=[O:25]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([CH2:6][CH2:7][CH2:8][O:9][Si:10]([CH3:11])([CH3:12])[C:13]([CH3:14])([CH3:15])[...
COC(=O)c1ccc(-c2ccc(CCCO[Si](C)(C)C(C)(C)C)cc2OC)cc1
COc1cc(CCCO[Si](C)(C)C(C)(C)C)ccc1-c1ccc(C(=O)O)cc1
null
null
C(C)(=O)OCC.C1CCOC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(-c2ccccc2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]
null
[]
null
null
3
HOUR
A mixture of Example 451A (828 mg, 2.0 mmol) and 1M LiOH (3 mL) in THF (10 mL) was heated to 50° C., stirred for 3 hours, diluted with ethyl acetate, washed with saturated sodium monobasic phosphate (10 mL), dried (MgSO4), filtered, and concentrated to provide the desired product. Conditions: See reaction.notes.procedu...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccccc1
Other
C(C)(=O)OCC.C1CCOC1
null
3
COC(=O)c1ccc(-c2ccc(CCCO[Si](C)(C)C(C)(C)C)cc2OC)cc1>C(C)(=O)OCC.C1CCOC1>COc1cc(CCCO[Si](C)(C)C(C)(C)C)ccc1-c1ccc(C(=O)O)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f393d314843f45daae93ff7e9eb80178
COC(=O)c1ccc(C2=CCN(C(=O)OC(C)(C)C)CC2)cc1.NS(=O)(=O)c1ccc(NCCSc2ccccc2)c([N+](=O)[O-])c1>>CC(C)(C)OC(=O)N1CC=C(c2ccc(C(=O)NS(=O)(=O)c3ccc(NCCSc4ccccc4)c([N+](=O)[O-])c3)cc2)CC1
[N+](=O)([O-])C=1C=C(C=CC1NCCSC1=CC=CC=C1)S(=O)(=O)N.CCN=C=NCCCN(C)C.COC(=O)C1=CC=C(C=C1)C=1CCN(CC1)C(=O)OC(C)(C)C.[Li+].[OH-]>>[N+](=O)([O-])C=1C=C(C=CC1NCCSC1=CC=CC=C1)S(=O)(=O)NC(=O)C1=CC=C(C=C1)C=1CCN(CC1)C(=O)OC(C)(C)C
CO[C:16]([c:15]1[cH:14][cH:13][c:12]([C:11]2=[CH:10][CH2:9][N:8]([C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[CH2:44][CH2:43]2)[cH:42][cH:41]1)=[O:17].[NH2:18][S:19](=[O:20])(=[O:21])[c:22]1[cH:23][cH:24][c:25]([NH:26][CH2:27][CH2:28][S:29][c:30]2[cH:31][cH:32][cH:33][cH:34][cH:35]2)[c:36]([N+:37](=[O:38])[O-:39])...
COC(=O)c1ccc(C2=CCN(C(=O)OC(C)(C)C)CC2)cc1.NS(=O)(=O)c1ccc(NCCSc2ccccc2)c([N+](=O)[O-])c1
CC(C)(C)OC(=O)N1CC=C(c2ccc(C(=O)NS(=O)(=O)c3ccc(NCCSc4ccccc4)c([N+](=O)[O-])c3)cc2)CC1
null
CN(C)C=1C=CN=CC1
O.C(C)(=O)OCC.ClC(C)Cl.CO.C1CCOC1
Acylation
Aminolysis of esters
5894ae7814242c4644e19aff394b08853b52e43b2f0bde0de031dced0ee91450
2dc8f17ecc2e722c5c3a62b720a5408c74a550fd92fbcd682ac09cdbc0305937
O=C(NS(=O)(=O)c1ccc(NCCSc2ccccc2)cc1)c1ccc(C2=CCNCC2)cc1
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[NH2;D1;+0:6]-[#16:7](=[O;D1;H0:8])(=[O;D1;H0:9])-[c:10]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[#16:7](=[O;D1;H0:8])(=[O;D1;H0:9])-[c:10])-[c:3](:[c:4]):[c:5]
null
[]
null
null
16
HOUR
A mixture of Example 455B (1 g, 3.1 mmol) and LiOH (0.264 mg 6.2 mmol) in THF (15 mL), methanol (2.5 mL), and water (1.5 mL) was heated to 50° C. for 3 hours and concentrated. The concentrate was dissolved in DMF (10 mL) and treated with a mixture of Example 77B (1.059 g, 3mmol), EDCI (1.146 g, 6 mmol), and DMAP (1.830...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Ester
Sulfonamide.Secondary amide
null
null
C1=CC[NH]CC1.c1ccccc1.c1ccccc1.c1ccccc1
HO-
CN(C)C=1C=CN=CC1.O.C(C)(=O)OCC.ClC(C)Cl.CO.C1CCOC1
null
16
COC(=O)c1ccc(C2=CCN(C(=O)OC(C)(C)C)CC2)cc1.NS(=O)(=O)c1ccc(NCCSc2ccccc2)c([N+](=O)[O-])c1>CN(C)C=1C=CN=CC1.O.C(C)(=O)OCC.ClC(C)Cl.CO.C1CCOC1>CC(C)(C)OC(=O)N1CC=C(c2ccc(C(=O)NS(=O)(=O)c3ccc(NCCSc4ccccc4)c([N+](=O)[O-])c3)cc2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-35b3679ab5b0449ea4e1d0eaec1f9fdb
N#C[O-].NCCCC[C@H](CSc1ccccc1)Nc1ccc(S(=O)(=O)NC(=O)c2ccc(N3CCC4(CCCC4)CC3)cc2)cc1[N+](=O)[O-]>>NC(=O)NCCCC[C@H](CSc1ccccc1)Nc1ccc(S(=O)(=O)NC(=O)c2ccc(N3CCC4(CCCC4)CC3)cc2)cc1[N+](=O)[O-]
NCCCC[C@H](CSC1=CC=CC=C1)NC1=C(C=C(C=C1)S(=O)(=O)NC(C1=CC=C(C=C1)N1CCC2(CCCC2)CC1)=O)[N+](=O)[O-].[O-]C#N.[K+].O>>NC(=O)NCCCC[C@H](CSC1=CC=CC=C1)NC1=C(C=C(C=C1)S(=O)(=O)NC(C1=CC=C(C=C1)N1CCC2(CCCC2)CC1)=O)[N+](=O)[O-]
[N:1]#[C:2][O-:3].[NH2:4][CH2:5][CH2:6][CH2:7][CH2:8][C@H:9]([CH2:10][S:11][c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1)[NH:18][c:19]1[cH:20][cH:21][c:22]([S:23](=[O:24])(=[O:25])[NH:26][C:27](=[O:28])[c:29]2[cH:30][cH:31][c:32]([N:33]3[CH2:34][CH2:35][C:36]4([CH2:37][CH2:38][CH2:39][CH2:40]4)[CH2:41][CH2:42]3)[cH:43][c...
N#C[O-].NCCCC[C@H](CSc1ccccc1)Nc1ccc(S(=O)(=O)NC(=O)c2ccc(N3CCC4(CCCC4)CC3)cc2)cc1[N+](=O)[O-]
NC(=O)NCCCC[C@H](CSc1ccccc1)Nc1ccc(S(=O)(=O)NC(=O)c2ccc(N3CCC4(CCCC4)CC3)cc2)cc1[N+](=O)[O-]
null
null
CO
Acylation
OtherReaction
f8798d1193af6f9b314ac8855e814716b90ff3758bcfa29778cc632fcaa83b7a
5efe06db19c806d9e9798893351dc14c0cc48f1e8f8c857f54c6171e86c96a1b
O=C(NS(=O)(=O)c1ccc(NCCSc2ccccc2)cc1)c1ccc(N2CCC3(CCCC3)CC2)cc1
[C:1]-[C:2]-[NH2;D1;+0:3].[N;H0;D1;+0:4]#[C;H0;D2;+0:5]-[O-;H0;D1:6]>>[C:1]-[C:2]-[NH;D2;+0:3]-[C;H0;D3;+0:5](-[NH2;D1;+0:4])=[O;H0;D1;+0:6]
null
[]
null
null
null
null
A solution of Example 287 (60 mg, 0.1 mmol) and potassium cyanate (20 mg, 0.25 mmol) in methanol (1 mL) was stirred at 55° C. for 1.5 hours, cooled to room temperature, treated with water, and extracted with dichloromethane. The combined extracts were washed with saturated sodium bicarbonate, dried (MgSO4), filtered, a...
10.6084/m9.figshare.5104873.v1
null
Nitrile.Primary amine
Urea
null
null
c1ccccc1.c1ccccc1.c1ccccc1.C1CCC2(C1)CC[NH]CC2
null
CO
null
null
N#C[O-].NCCCC[C@H](CSc1ccccc1)Nc1ccc(S(=O)(=O)NC(=O)c2ccc(N3CCC4(CCCC4)CC3)cc2)cc1[N+](=O)[O-]>CO>NC(=O)NCCCC[C@H](CSc1ccccc1)Nc1ccc(S(=O)(=O)NC(=O)c2ccc(N3CCC4(CCCC4)CC3)cc2)cc1[N+](=O)[O-]
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-244e338b6ba5467ab1f9666d165202d8
CC(C)(C)OC(=O)/C=C/[C@H](CSc1ccccc1)NC(=O)OC(C)(C)C>>CC(C)(C)OC(=O)N[C@H](CCC(=O)O)CSc1ccccc1
C(C)(C)(C)OC(=O)N[C@H](/C=C/C(=O)OC(C)(C)C)CSC1=CC=CC=C1>>C(C)(C)(C)OC(=O)N[C@H](CCC(=O)O)CSC1=CC=CC=C1
CC(C)(C)[O:14][C:12](/[CH:11]=[CH:10]/[C@@H:9]([NH:8][C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[CH2:15][S:16][c:17]1[cH:18][cH:19][cH:20][cH:21][cH:22]1)=[O:13]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[NH:8][C@H:9]([CH2:10][CH2:11][C:12](=[O:13])[OH:14])[CH2:15][S:16][c:17]1[cH:18][cH:19][cH:20][cH:21][...
CC(C)(C)OC(=O)/C=C/[C@H](CSc1ccccc1)NC(=O)OC(C)(C)C
CC(C)(C)OC(=O)N[C@H](CCC(=O)O)CSc1ccccc1
null
C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.[Cl-].[Rh]
null
Deprotection
OtherReaction
152e5537e48c95b4a3e767536b0f9f68d1308e5f484070828ab5ed951805157a
7f019d4cfe9b3036d0a2d3a3209aa0e1fcb05418ebee15a4be5e125d315d5f01
c1ccccc1
C-C(-C)(-C)-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])/[CH;D2;+0:4]=[CH;D2;+0:5]/[C:6](-[C:7])-[#7:8]-[C:9](=[O;D1;H0:10])-[#8:11]-[C:12](-[C;D1;H3:13])(-[C;D1;H3:14])-[C;D1;H3:15]>>[C:7]-[C:6](-[#7:8]-[C:9](=[O;D1;H0:10])-[#8:11]-[C:12](-[C;D1;H3:13])(-[C;D1;H3:14])-[C;D1;H3:15])-[CH2;D2;+0:5]-[CH2;D2;+0:4]-[C:2](=[O;D1;H0:3]...
null
[]
null
null
24
HOUR
A mixture of Example 480A (5 g, 13.2 mmol) and Wilkinson's catalyst (1 g) in tolune (125 mL) was stirred under H2at 60° C. for 18 hours, cooled, filtered through silica gel, and concentrated. The concentrate was dissolved in 3:1:1 THF/water/MeOH (150 mL), treated with with a 10-fold excess of LiOH, and stirred for 24 h...
10.6084/m9.figshare.5104873.v1
null
Ester.Boc
Carboxylic acid
null
null
c1ccccc1
Other
C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.[Cl-].[Rh]
null
24
CC(C)(C)OC(=O)/C=C/[C@H](CSc1ccccc1)NC(=O)OC(C)(C)C>C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.[Cl-].[Rh]>CC(C)(C)OC(=O)N[C@H](CCC(=O)O)CSc1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-bd546c45247d43fb9d71ec8beb332979
COC(=O)c1ccc(-c2ccc(CCO)cc2OC)cc1>>COC(=O)c1ccc(-c2ccc(CC=O)cc2OC)cc1
OCCC1=CC(=C(C=C1)C1=CC=C(C=C1)C(=O)OC)OC.CC(=O)OI1(C=2C=CC=CC2C(=O)O1)(OC(=O)C)OC(=O)C>>COC1=C(C=CC(=C1)CC=O)C1=CC=C(C=C1)C(=O)OC
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8](-[c:9]2[cH:10][cH:11][c:12]([CH2:13][CH2:14][OH:15])[cH:16][c:17]2[O:18][CH3:19])[cH:20][cH:21]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8](-[c:9]2[cH:10][cH:11][c:12]([CH2:13][CH:14]=[O:15])[cH:16][c:17]2[O:18][CH3:19])[cH:20][cH:21]1
COC(=O)c1ccc(-c2ccc(CCO)cc2OC)cc1
COC(=O)c1ccc(-c2ccc(CC=O)cc2OC)cc1
null
null
ClCCl
Oxidation
Oxidation or Dehydrogenation of Alcohols to Aldehydes and Ketones
41bfa9deea81b465c88ad21fdfb64a2e1ba29490558cf430df132cb98b4a538b
0a03c6724c1862e8f86d4a463afda55b8e067dc6cb42597b472eb7cabc03eda3
c1ccc(-c2ccccc2)cc1
[OH;D1;+0:1]-[CH2;D2;+0:2]-[C:3]-[c:4]>>[O;H0;D1;+0:1]=[CH;D2;+0:2]-[C:3]-[c:4]
null
[]
null
null
90
MINUTE
A solution of Example 491B (2.47 g, 8.63 mmol) in dichloromethane (25 mL) at room temperature was treated with Dess-Martin periodinane (4.03 g, 9.49 mmol), stirred for 90 minutes, and concentrated The concentrate was purified by flash column chromatography on silica gel with 1:1 ethyl acetate/hexanes to provide the des...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Aldehyde
null
null
c1ccccc1.c1ccccc1
null
ClCCl
null
1.5
COC(=O)c1ccc(-c2ccc(CCO)cc2OC)cc1>ClCCl>COC(=O)c1ccc(-c2ccc(CC=O)cc2OC)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-463b713c69c341fd8ab16bd434ac5757
CC(C)(C)OC(=O)N1CCNCC1.COC(=O)c1ccc(-c2ccc(CC=O)cc2OC)cc1>>COC(=O)c1ccc(-c2ccc(CCN3CCN(C(=O)OC(C)(C)C)CC3)cc2OC)cc1
COC1=C(C=CC(=C1)CC=O)C1=CC=C(C=C1)C(=O)OC.N1(CCNCC1)C(=O)OC(C)(C)C.C(C)(=O)O[BH-](OC(C)=O)OC(C)=O.[Na+]>>COC1=C(C=CC(=C1)CCN1CCN(CC1)C(=O)OC(C)(C)C)C1=CC=C(C=C1)C(=O)OC
[NH:15]1[CH2:16][CH2:17][N:18]([C:19](=[O:20])[O:21][C:22]([CH3:23])([CH3:24])[CH3:25])[CH2:26][CH2:27]1.O=[CH:14][CH2:13][c:12]1[cH:11][cH:10][c:9](-[c:8]2[cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:33][cH:32]2)[c:29]([O:30][CH3:31])[cH:28]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8](-[c:9]2[cH:10][cH:11][c...
CC(C)(C)OC(=O)N1CCNCC1.COC(=O)c1ccc(-c2ccc(CC=O)cc2OC)cc1
COC(=O)c1ccc(-c2ccc(CCN3CCN(C(=O)OC(C)(C)C)CC3)cc2OC)cc1
null
null
ClCCCl
Heteroatom Alkylation and Arylation
reductive amination
7a1842565a3c73c1d6bba5dccafef60d48e9eaf6e4a0871f60e828bcbdf26fb1
2d03f38884b1fbb0c0d6e6f2de31afb25102fec87f347c3a123e064c1bfef0ad
c1ccc(-c2ccc(CCN3CCNCC3)cc2)cc1
O=[CH;D2;+0:1]-[C:2]-[c:3].[#7:4]1-[C:5]-[C:6]-[NH;D2;+0:7]-[C:8]-[C:9]-1>>[c:3]-[C:2]-[CH2;D2;+0:1]-[N;H0;D3;+0:7]1-[C:6]-[C:5]-[#7:4]-[C:9]-[C:8]-1
null
[]
null
null
16
HOUR
A solution of Example 491C (400 mg, 1.41 mmol) and tert-butyl 1-piperazinecarboxylate (289 mg, 1.55 mmol) in 1,2-dichloroethane (5mL) at room temperature was treated with sodium triacetoxyborohydride (329 mg, 1.55 mmol), and stirred for 16 hours. The solution was purified by flash column chromatography on silica gel wi...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Secondary amine
Tertiary amine
C1CNCC[NH]1
C1C[NH]CC[NH]1
c1ccccc1.c1ccccc1.C1C[NH]CC[NH]1
Other
ClCCCl
null
16
CC(C)(C)OC(=O)N1CCNCC1.COC(=O)c1ccc(-c2ccc(CC=O)cc2OC)cc1>ClCCCl>COC(=O)c1ccc(-c2ccc(CCN3CCN(C(=O)OC(C)(C)C)CC3)cc2OC)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6e76420ede2d46449fa7caf17eec7309
CC(C)(C)OC(=O)c1ccc(F)cc1.OC1(c2ccccc2)CCNCC1>>CC(C)(C)OC(=O)c1ccc(N2CCC(O)(c3ccccc3)CC2)cc1
OC1(CCNCC1)C1=CC=CC=C1.C(C)(C)(C)OC(C1=CC=C(C=C1)F)=O.C([O-])([O-])=O.[K+].[K+]>>OC1(CCN(CC1)C1=CC=C(C(=O)OC(C)(C)C)C=C1)C1=CC=CC=C1
F[c:11]1[cH:10][cH:9][c:8]([C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[cH:26][cH:25]1.[NH:12]1[CH2:13][CH2:14][C:15]([OH:16])([c:17]2[cH:18][cH:19][cH:20][cH:21][cH:22]2)[CH2:23][CH2:24]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[c:8]1[cH:9][cH:10][c:11]([N:12]2[CH2:13][CH2:14][C:15]([OH:16])([c:17]3[cH:1...
CC(C)(C)OC(=O)c1ccc(F)cc1.OC1(c2ccccc2)CCNCC1
CC(C)(C)OC(=O)c1ccc(N2CCC(O)(c3ccccc3)CC2)cc1
null
null
CS(=O)C.C(C)OCC
Heteroatom Alkylation and Arylation
Buchwald-Hartwig/Ullmann-Goldberg/N-arylation secondary amine
ad5ec9c4592e4dee5877fc4f1309a503a378773e18ebc21adf780b709f6e28c5
b6b8e2cdb45054a35f5e8157d624f852c0601a09401556706e166b19536eb7a7
c1ccc(C2CCN(c3ccccc3)CC2)cc1
F-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[C:6]-[C:7]-[NH;D2;+0:8]-[C:9]-[C:10]>>[C:6]-[C:7]-[N;H0;D3;+0:8](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5])-[C:9]-[C:10]
null
[]
125
CELSIUS
16
HOUR
A solution of 4-hydroxy-4-phenyl piperidine (221 mg, 1.25 mmol) in DMSO (1 mL) was treated with tert-butyl-4-fluorobenzoate (196 mg, 1.00 mmol) and powdered potassium carbonate (173 mg, 1.25 mmol), stirred vigorously at 125° C. for 16 hours, cooled to room temperature, diluted with diethyl ether, washed with brine, dri...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Secondary amine
Tertiary amine
c1ccccc1.C1CCNCC1
c1ccccc1.C1CC[NH]CC1
c1ccccc1.C1CC[NH]CC1.c1ccccc1
HF
CS(=O)C.C(C)OCC
125
16
CC(C)(C)OC(=O)c1ccc(F)cc1.OC1(c2ccccc2)CCNCC1>CS(=O)C.C(C)OCC>CC(C)(C)OC(=O)c1ccc(N2CCC(O)(c3ccccc3)CC2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9d85b669c2214a29b20c5d1fbbd89044
CC(C)(C)OC(=O)c1ccc(N2CCC(O)(c3ccccc3)CC2)cc1>>O=C(O)c1ccc(N2CCC(O)(c3ccccc3)CC2)cc1
OC1(CCN(CC1)C1=CC=C(C(=O)OC(C)(C)C)C=C1)C1=CC=CC=C1>>OC1(CCN(CC1)C1=CC=C(C(=O)O)C=C1)C1=CC=CC=C1
CC(C)(C)[O:3][C:2](=[O:1])[c:4]1[cH:5][cH:6][c:7]([N:8]2[CH2:9][CH2:10][C:11]([OH:12])([c:13]3[cH:14][cH:15][cH:16][cH:17][cH:18]3)[CH2:19][CH2:20]2)[cH:21][cH:22]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][c:7]([N:8]2[CH2:9][CH2:10][C:11]([OH:12])([c:13]3[cH:14][cH:15][cH:16][cH:17][cH:18]3)[CH2:19][CH2:20]2)[cH:21][cH:2...
CC(C)(C)OC(=O)c1ccc(N2CCC(O)(c3ccccc3)CC2)cc1
O=C(O)c1ccc(N2CCC(O)(c3ccccc3)CC2)cc1
null
null
C(=O)(C(F)(F)F)O
Deprotection
Deprotection of carboxylic acid
152e5537e48c95b4a3e767536b0f9f68d1308e5f484070828ab5ed951805157a
7f019d4cfe9b3036d0a2d3a3209aa0e1fcb05418ebee15a4be5e125d315d5f01
c1ccc(C2CCN(c3ccccc3)CC2)cc1
C-C(-C)(-C)-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]
null
[]
null
null
null
null
A solution of Example 493A (0.32 g, 0.91 mmol) in TFA (2 mL) at room temperature was stirred for 1 hour, and concentrated. The concentrate was azeotropically distilled with toluene three times and dried to provide the desired product. MS (ESI(+)) m/e 298 (M+H)+. Conditions: See reaction.notes.procedure_details. Workup:...
10.6084/m9.figshare.5104873.v1
null
Ester.Boc
Carboxylic acid
null
null
c1ccccc1.C1CC[NH]CC1.c1ccccc1
Other
C(=O)(C(F)(F)F)O
null
null
CC(C)(C)OC(=O)c1ccc(N2CCC(O)(c3ccccc3)CC2)cc1>C(=O)(C(F)(F)F)O>O=C(O)c1ccc(N2CCC(O)(c3ccccc3)CC2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6fc64735f1c047d6841d9d765cf70abe
CC(C)(C)OC(=O)N1CCC(=O)CC1>>CC1(O)CCN(C(=O)OC(C)(C)C)CC1
C[Mg]Br.O=C1CCN(CC1)C(=O)OC(C)(C)C.[NH4+].[Cl-]>>OC1(CCN(CC1)C(=O)OC(C)(C)C)C
[C:2]1(=[O:3])[CH2:4][CH2:5][N:6]([C:7](=[O:8])[O:9][C:10]([CH3:11])([CH3:12])[CH3:13])[CH2:14][CH2:15]1>>[CH3:1][C:2]1([OH:3])[CH2:4][CH2:5][N:6]([C:7](=[O:8])[O:9][C:10]([CH3:11])([CH3:12])[CH3:13])[CH2:14][CH2:15]1
CC(C)(C)OC(=O)N1CCC(=O)CC1
CC1(O)CCN(C(=O)OC(C)(C)C)CC1
null
null
C(C)OCC
Miscellaneous
OtherReaction
dfefed99c59b497159616052101f24c8ee451a3c3938a028396dd346c800e3a6
8811b4d793f7cfa9f0f1f47a008648edabb54f371f76dfa680dd5b2e1564c6c5
C1CCNCC1
[O;H0;D1;+0:1]=[C;H0;D3;+0:2]1-[C:3]-[C:4]-[#7:5]-[C:6]-[C:7]-1>>[C;D1;H3:8]-[C;H0;D4;+0:2]1(-[OH;D1;+0:1])-[C:3]-[C:4]-[#7:5]-[C:6]-[C:7]-1
null
[]
null
null
18
HOUR
A solution of 3M methyl magnesium bromide in diethyl ether (2.0 mL) in diethyl ether (3 mL) at 0° C. was treated with a solution of tert-butyl 4-oxo-1-piperidinecarboxylate (1.0 g, 5.00 mmol) in diethyl ether (5 mL), warmed to room temperature, stirred for 18 hours, treated with saturated NH4Cl, and extracted with diet...
10.6084/m9.figshare.5104873.v1
null
Ketone
Tertiary alcohol
C1CC[NH]CC1
C1CC[NH]CC1
C1CC[NH]CC1
Other
C(C)OCC
null
18
CC(C)(C)OC(=O)N1CCC(=O)CC1>C(C)OCC>CC1(O)CCN(C(=O)OC(C)(C)C)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-72f9d7eccb6240f287d432ceb20a86d6
COc1cc(CCN2CCN(C(=O)OC(C)(C)C)CC2)ccc1-c1ccc(C(=O)NS(=O)(=O)c2ccc(N[C@H](CCN(C)C)CSc3ccccc3)c([N+](=O)[O-])c2)cc1>>COc1cc(CCN2CCNCC2)ccc1-c1ccc(C(=O)NS(=O)(=O)c2ccc(N[C@H](CCN(C)C)CSc3ccccc3)c([N+](=O)[O-])c2)cc1
CN(CC[C@H](CSC1=CC=CC=C1)NC1=C(C=C(C=C1)S(=O)(=O)NC(=O)C1=CC=C(C=C1)C1=C(C=C(C=C1)CCN1CCN(CC1)C(=O)OC(C)(C)C)OC)[N+](=O)[O-])C>>CN(CC[C@H](CSC1=CC=CC=C1)NC1=C(C=C(C=C1)S(=O)(=O)NC(=O)C1=CC=C(C=C1)C1=C(C=C(C=C1)CCN1CCNCC1)OC)[N+](=O)[O-])C
CC(C)(C)OC(=O)[N:11]1[CH2:10][CH2:9][N:8]([CH2:7][CH2:6][c:5]2[cH:4][c:3]([O:2][CH3:1])[c:16](-[c:17]3[cH:18][cH:19][c:20]([C:21](=[O:22])[NH:23][S:24](=[O:25])(=[O:26])[c:27]4[cH:28][cH:29][c:30]([NH:31][C@H:32]([CH2:33][CH2:34][N:35]([CH3:36])[CH3:37])[CH2:38][S:39][c:40]5[cH:41][cH:42][cH:43][cH:44][cH:45]5)[c:46]([...
COc1cc(CCN2CCN(C(=O)OC(C)(C)C)CC2)ccc1-c1ccc(C(=O)NS(=O)(=O)c2ccc(N[C@H](CCN(C)C)CSc3ccccc3)c([N+](=O)[O-])c2)cc1
COc1cc(CCN2CCNCC2)ccc1-c1ccc(C(=O)NS(=O)(=O)c2ccc(N[C@H](CCN(C)C)CSc3ccccc3)c([N+](=O)[O-])c2)cc1
null
null
O1CCOCC1.Cl
Reduction
Boc amine deprotection
2c25e19aee181a3c5131cfdfda27035fd54d4379a11d745dfb75d386bacfd500
a94b29c7264c852156fc1cdd4a0951a4fc26c06d0edc9e50c743825dbf79e3fd
O=C(NS(=O)(=O)c1ccc(NCCSc2ccccc2)cc1)c1ccc(-c2ccc(CCN3CCNCC3)cc2)cc1
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1]1-[C:2]-[C:3]-[#7:4]-[C:5]-[C:6]-1>>[#7:4]1-[C:5]-[C:6]-[NH;D2;+0:1]-[C:2]-[C:3]-1
null
[]
null
null
null
null
A solution of Example 491F (284 mg, 0.34 mmol) in 1,4-dioxane (1.5 mL) and 4M HCl (1.5 mL) at room temperature was stirred for 16 hours. The solution was purified by flash column chromatography on silica gel with 80:20:0.5 dichloromethane/methanol/concentrated ammonium hydroxide to provide the desired product. MS (ESI)...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Secondary amine
C1C[NH]CC[NH]1
C1C[NH]CCN1
c1ccccc1.C1C[NH]CCN1.c1ccccc1.c1ccccc1.c1ccccc1
HO-
O1CCOCC1.Cl
null
null
COc1cc(CCN2CCN(C(=O)OC(C)(C)C)CC2)ccc1-c1ccc(C(=O)NS(=O)(=O)c2ccc(N[C@H](CCN(C)C)CSc3ccccc3)c([N+](=O)[O-])c2)cc1>O1CCOCC1.Cl>COc1cc(CCN2CCNCC2)ccc1-c1ccc(C(=O)NS(=O)(=O)c2ccc(N[C@H](CCN(C)C)CSc3ccccc3)c([N+](=O)[O-])c2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d68fb9f122fd402c93a8c8a38a6587a0
CC(C)(C)OC(=O)OC(=O)OC(C)(C)C.O=C1CNCCN1>>CC(C)(C)OC(=O)N1CCNC(=O)C1
N1C(CNCC1)=O.O(C(=O)OC(C)(C)C)C(=O)OC(C)(C)C>>O=C1CN(CCN1)C(=O)OC(C)(C)C
CC(C)(C)OC(=O)O[C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7].[NH:8]1[CH2:9][CH2:10][NH:11][C:12](=[O:13])[CH2:14]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[N:8]1[CH2:9][CH2:10][NH:11][C:12](=[O:13])[CH2:14]1
CC(C)(C)OC(=O)OC(=O)OC(C)(C)C.O=C1CNCCN1
CC(C)(C)OC(=O)N1CCNC(=O)C1
null
null
C(C)#N
Protection
Boc amine protection with Boc anhydride
6b6bceeda760b13c0e0d3785668f44a028e616c30bc5b09d93a2450415ad5022
7c9d9ba915c29b1020a278f50f3c8f9cc1fd09ebab5bff22f0c1b047d4ae169a
O=C1CNCCN1
C-C(-C)(-C)-O-C(=O)-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C:4](-[C;D1;H3:5])(-[C;D1;H3:6])-[C;D1;H3:7].[O;D1;H0:8]=[C:9]1-[#7:10]-[C:11]-[C:12]-[NH;D2;+0:13]-[C:14]-1>>[C;D1;H3:5]-[C:4](-[C;D1;H3:6])(-[C;D1;H3:7])-[#8:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[N;H0;D3;+0:13]1-[C:14]-[C:9](=[O;D1;H0:8])-[#7:10]-[C:11]-[C:12]-1
null
[]
null
null
3
HOUR
A solution of Example 500A (500 mg, 4.99 mmol) in acetonitrile (25 mL) at room temperature was treated with BOC2O (1198 mg, 5.49 mmol), stirred for 3 hours, and concentrated. The concentrate was purified by flash column chromatography on silica gel with 95:5 ethyl acetate/methanol to provide the desired product. Condit...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Carbonic Ester.Carbonic Ester.Secondary amine.Boc.Boc
Carbamic ester
C1CNCCN1
C1C[NH]CCN1
C1C[NH]CCN1
HO-
C(C)#N
null
3
CC(C)(C)OC(=O)OC(=O)OC(C)(C)C.O=C1CNCCN1>C(C)#N>CC(C)(C)OC(=O)N1CCNC(=O)C1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-39c52997c4d64128b0ec907743324cfd
C=CCOC1(CC=C)CCN(C(=O)OC(C)(C)C)CC1>>CC(C)(C)OC(=O)N1CCC2(CC=CCO2)CC1
C(C=C)C1(CCN(CC1)C(=O)OC(C)(C)C)OCC=C>>O1CC=CCC12CCN(CC2)C(=O)OC(C)(C)C
C=[CH:13][CH2:12][C:11]1([O:16][CH2:15][CH:14]=C)[CH2:10][CH2:9][N:8]([C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[CH2:18][CH2:17]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[N:8]1[CH2:9][CH2:10][C:11]2([CH2:12][CH:13]=[CH:14][CH2:15][O:16]2)[CH2:17][CH2:18]1
C=CCOC1(CC=C)CCN(C(=O)OC(C)(C)C)CC1
CC(C)(C)OC(=O)N1CCC2(CC=CCO2)CC1
null
null
C1=CC=CC=C1
C-C Coupling
OtherReaction
ce2b403338073b1a94caab8e44a26ee04764997d0593da03d3176d1f623e82cf
67a23c4de67c22dcd6bc1d4c033efdcf679af248440c3b10e6768679c5f73280
C1=CCC2(CCNCC2)OC1
C=[CH;D2;+0:1]-[C:2]-[C:3]-[#8:4]-[C:5]-[CH;D2;+0:6]=C>>[#8:4]1-[C:3]-[C:2]-[CH;D2;+0:1]=[CH;D2;+0:6]-[C:5]-1
null
[]
null
null
18
HOUR
A solution of Example 518B (0.79 g, 2.81 mmol) in degassed benzene (100 mL) at room temperature was treated with bis-tricyclohexylphosphine benzylidene ruthenium (IV) dichloride (150 mg), stirred for 18 hours, and concentrated The concentrate was purified by flash column chromatography on silica gel with 10%-25% ethyl ...
10.6084/m9.figshare.5104873.v1
null
Allyl.Allyl
null
null
C1=CCC2(CC[NH]CC2)OC1
C1=CCC2(CC[NH]CC2)OC1
Other
C1=CC=CC=C1
null
18
C=CCOC1(CC=C)CCN(C(=O)OC(C)(C)C)CC1>C1=CC=CC=C1>CC(C)(C)OC(=O)N1CCC2(CC=CCO2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ce224a7eabf04ad5997f3efe1cb72212
CCOC(=O)C1CCN(C(=O)OC(C)(C)C)CC1.CI>>CCOC(=O)C1(C)CCN(C(=O)OC(C)(C)C)CC1
CI.N1(CCC(CC1)C(=O)OCC)C(=O)OC(C)(C)C.[Li+].CC(C)[N-]C(C)C.C1CCCCC1>>CC1(CCN(CC1)C(=O)OC(C)(C)C)C(=O)OCC
[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]1[CH2:8][CH2:9][N:10]([C:11](=[O:12])[O:13][C:14]([CH3:15])([CH3:16])[CH3:17])[CH2:18][CH2:19]1.I[CH3:7]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[C:6]1([CH3:7])[CH2:8][CH2:9][N:10]([C:11](=[O:12])[O:13][C:14]([CH3:15])([CH3:16])[CH3:17])[CH2:18][CH2:19]1
CCOC(=O)C1CCN(C(=O)OC(C)(C)C)CC1.CI
CCOC(=O)C1(C)CCN(C(=O)OC(C)(C)C)CC1
null
null
C1CCOC1
C-C Coupling
Methylation with MeI_tertiary
6bdbd896659a1d85611ac4aba77b405f65bed934821cffd10e318213ab724706
49d6f28766066d07dffbcc6f4da77792f6ba67b4de619800bad651525d6fe2e7
C1CCNCC1
I-[CH3;D1;+0:1].[C:2]-[#8:3]-[C:4](=[O;D1;H0:5])-[CH;D3;+0:6]1-[C:7]-[C:8]-[#7:9]-[C:10]-[C:11]-1>>[C:2]-[#8:3]-[C:4](=[O;D1;H0:5])-[C;H0;D4;+0:6]1(-[CH3;D1;+0:1])-[C:7]-[C:8]-[#7:9]-[C:10]-[C:11]-1
null
[]
null
null
30
MINUTE
A solution of Example 532A (2.1 g, 8.1 mmol) in THF (81 mL) at −78° C. was treated dropwise with 1.5M LDA in cyclohexane (6.0 mL, 8.9 mmol), stirred for 30 minutes, treated dropwise with methyl iodide (0.76 mL, 12.1 mmol), stirred for 2.5 hours, quenched with saturated NH4Cl, and extracted with diethyl ether. The combi...
10.6084/m9.figshare.5104873.v1
null
Ester
Ester
C1CC[NH]CC1
C1CC[NH]CC1
C1CC[NH]CC1
HI
C1CCOC1
null
0.5
CCOC(=O)C1CCN(C(=O)OC(C)(C)C)CC1.CI>C1CCOC1>CCOC(=O)C1(C)CCN(C(=O)OC(C)(C)C)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c9a185424ee24b58b45040fed79c6a82
CCOC(=O)C1(C)CCN(C(=O)OC(C)(C)C)CC1>>CCOC(=O)C1(C)CCNCC1
CC1(CCN(CC1)C(=O)OC(C)(C)C)C(=O)OCC>>CC1(CCNCC1)C(=O)OCC
CC(C)(C)OC(=O)[N:10]1[CH2:9][CH2:8][C:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])([CH3:7])[CH2:12][CH2:11]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[C:6]1([CH3:7])[CH2:8][CH2:9][NH:10][CH2:11][CH2:12]1
CCOC(=O)C1(C)CCN(C(=O)OC(C)(C)C)CC1
CCOC(=O)C1(C)CCNCC1
null
null
Cl.O1CCOCC1
Reduction
Boc amine deprotection
bf3cd5dc3e17e694d8665c89f5d7e08e8763b18436a633eb66e9bf530b8b0316
a94b29c7264c852156fc1cdd4a0951a4fc26c06d0edc9e50c743825dbf79e3fd
C1CCNCC1
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1](-[C:2]-[C:3])-[C:4]-[C:5]>>[C:3]-[C:2]-[NH;D2;+0:1]-[C:4]-[C:5]
null
[]
null
null
null
null
A solution of Example 532B (2.1 g, 8.0 mmol) in 4M HCl in dioxane (10 mL) at room temperature was stirred for 3 hours and concentrated to provide the desired product. MS (DCI) mne 171 (M+H)+. Conditions: See reaction.notes.procedure_details. Workup: concentrated
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Secondary amine
C1CC[NH]CC1
C1CCNCC1
C1CCNCC1
HO-
Cl.O1CCOCC1
null
null
CCOC(=O)C1(C)CCN(C(=O)OC(C)(C)C)CC1>Cl.O1CCOCC1>CCOC(=O)C1(C)CCNCC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-13c4913959d247738f507fd2a658886d
BrCc1ccccc1.O=C(O)c1ccc(F)cc1>>O=C(OCc1ccccc1)c1ccc(F)cc1
FC1=CC=C(C(=O)O)C=C1.C(C1=CC=CC=C1)Br.C([O-])([O-])=O.[Cs+].[Cs+]>>FC1=CC=C(C(=O)OCC2=CC=CC=C2)C=C1
Br[CH2:4][c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1.[O:1]=[C:2]([OH:3])[c:11]1[cH:12][cH:13][c:14]([F:15])[cH:16][cH:17]1>>[O:1]=[C:2]([O:3][CH2:4][c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1)[c:11]1[cH:12][cH:13][c:14]([F:15])[cH:16][cH:17]1
BrCc1ccccc1.O=C(O)c1ccc(F)cc1
O=C(OCc1ccccc1)c1ccc(F)cc1
null
null
O.CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
06c4f868ad4646eea8208ecb83f54ca035dd62d04f0d8101641a4f487f2c695c
8446834f0edd1e71a2dcaffc09b80c7367abf3407263a8998354a2d20c1766bb
O=C(OCc1ccccc1)c1ccccc1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[O;D1;H0:5]=[C:6](-[OH;D1;+0:7])-[c:8]>>[O;D1;H0:5]=[C:6](-[c:8])-[O;H0;D2;+0:7]-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
24
HOUR
A mixture of 4-fluorobenzoic acid (4.9 g, 35.3 mmol), benzyl bromide (3.8 mL, 31.7 mmol), and cesium carbonate (17.2 g, 53 mmol) in DMF (50 mL,) at room temperature was stirred for 24 hours, diluted with water, and extracted with diethyl ether. The combined extracts were washed with brine, dried (MgSO4), filtered, and ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Carboxylic acid
Ester
null
null
c1ccccc1.c1ccccc1
HBr
O.CN(C)C=O
null
24
BrCc1ccccc1.O=C(O)c1ccc(F)cc1>O.CN(C)C=O>O=C(OCc1ccccc1)c1ccc(F)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5ac43e5e93c54008ba4c942b6b3598b4
CC1(C(=O)O)CCN(c2ccc(C(=O)NS(=O)(=O)c3ccc(NCCSc4ccccc4)c([N+](=O)[O-])c3)cc2)CC1>>CC1(CO)CCN(c2ccc(C(=O)NS(=O)(=O)c3ccc(NCCSc4ccccc4)c([N+](=O)[O-])c3)cc2)CC1
[BH4-].[Na+].CC1(CCN(CC1)C1=CC=C(C=C1)C(=O)NS(=O)(=O)C1=CC(=C(C=C1)NCCSC1=CC=CC=C1)[N+](=O)[O-])C(=O)O.CN1CCOCC1.ClC(=O)OCC(C)C>>OCC1(CCN(CC1)C1=CC=C(C(=O)NS(=O)(=O)C2=CC(=C(C=C2)NCCSC2=CC=CC=C2)[N+](=O)[O-])C=C1)C
O=[C:3]([C:2]1([CH3:1])[CH2:5][CH2:6][N:7]([c:8]2[cH:9][cH:10][c:11]([C:12](=[O:13])[NH:14][S:15](=[O:16])(=[O:17])[c:18]3[cH:19][cH:20][c:21]([NH:22][CH2:23][CH2:24][S:25][c:26]4[cH:27][cH:28][cH:29][cH:30][cH:31]4)[c:32]([N+:33](=[O:34])[O-:35])[cH:36]3)[cH:37][cH:38]2)[CH2:39][CH2:40]1)[OH:4]>>[CH3:1][C:2]1([CH2:3][...
CC1(C(=O)O)CCN(c2ccc(C(=O)NS(=O)(=O)c3ccc(NCCSc4ccccc4)c([N+](=O)[O-])c3)cc2)CC1
CC1(CO)CCN(c2ccc(C(=O)NS(=O)(=O)c3ccc(NCCSc4ccccc4)c([N+](=O)[O-])c3)cc2)CC1
null
null
O.COCCOC
Reduction
Reduction of carboxylic acid to primary alcohol
0db83a5ebe1e318b78b55461cf7eb8f7c004eef0f9e3b6666d3df4c96b5f665e
93b4621647b04d2ad2f2825215b1567f171ba61fe10d136b5db6ea0470aa4932
O=C(NS(=O)(=O)c1ccc(NCCSc2ccccc2)cc1)c1ccc(N2CCCCC2)cc1
O=[C;H0;D3;+0:1](-[O;D1;H1:2])-[C:3](-[C;D1;H3:4])(-[C:5])-[C:6]>>[C:5]-[C:3](-[C;D1;H3:4])(-[CH2;D2;+0:1]-[O;D1;H1:2])-[C:6]
null
[]
-15
CELSIUS
15
MINUTE
A solution of Example 532H (35 mg, 0.06 mmol), 4-methylmorpholine (0.007 mL, 0.06 mmol), and DME (0.3 mL) at −15° C. was treated dropwise with isobutyl chloroformate (0.008 mL, 0.06 mmol), stirred for 15 minutes, and filtered. The filter cake was washed with DME and the filtrate and washings were combined. The solution...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Primary alcohol
null
null
C1CC[NH]CC1.c1ccccc1.c1ccccc1.c1ccccc1
Other
O.COCCOC
-15
0.25
CC1(C(=O)O)CCN(c2ccc(C(=O)NS(=O)(=O)c3ccc(NCCSc4ccccc4)c([N+](=O)[O-])c3)cc2)CC1>O.COCCOC>CC1(CO)CCN(c2ccc(C(=O)NS(=O)(=O)c3ccc(NCCSc4ccccc4)c([N+](=O)[O-])c3)cc2)CC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f6782bcb88384b5ca2b69805ae1eddde
NCCCC[C@H](CSc1ccccc1)Nc1ccc(S(=O)(=O)NC(=O)c2ccc(N3CCC4(CCCC4)CC3)cc2)cc1[N+](=O)[O-]>>N=C(N)NCCCC[C@H](CSc1ccccc1)Nc1ccc(S(=O)(=O)NC(=O)c2ccc(N3CCC4(CCCC4)CC3)cc2)cc1[N+](=O)[O-]
NCCCC[C@H](CSC1=CC=CC=C1)NC1=C(C=C(C=C1)S(=O)(=O)NC(C1=CC=C(C=C1)N1CCC2(CCCC2)CC1)=O)[N+](=O)[O-].C(C)(C)N(CC)C(C)C.CN(C)C=O>>NC(=N)NCCCC[C@H](CSC1=CC=CC=C1)NC1=C(C=C(C=C1)S(=O)(=O)NC(C1=CC=C(C=C1)N1CCC2(CCCC2)CC1)=O)[N+](=O)[O-]
[NH2:4][CH2:5][CH2:6][CH2:7][CH2:8][C@H:9]([CH2:10][S:11][c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1)[NH:18][c:19]1[cH:20][cH:21][c:22]([S:23](=[O:24])(=[O:25])[NH:26][C:27](=[O:28])[c:29]2[cH:30][cH:31][c:32]([N:33]3[CH2:34][CH2:35][C:36]4([CH2:37][CH2:38][CH2:39][CH2:40]4)[CH2:41][CH2:42]3)[cH:43][cH:44]2)[cH:45][c:4...
NCCCC[C@H](CSc1ccccc1)Nc1ccc(S(=O)(=O)NC(=O)c2ccc(N3CCC4(CCCC4)CC3)cc2)cc1[N+](=O)[O-]
N=C(N)NCCCC[C@H](CSc1ccccc1)Nc1ccc(S(=O)(=O)NC(=O)c2ccc(N3CCC4(CCCC4)CC3)cc2)cc1[N+](=O)[O-]
null
null
null
Functional Group Addition
OtherReaction
4fbd61810687f265a1928bdad0d611b8a3b0a276707821eb7e74c90a9b8fe484
c15d00b2143ff6be17711701b3a1268fe1c3598f83b20a6cd29a72406090607e
O=C(NS(=O)(=O)c1ccc(NCCSc2ccccc2)cc1)c1ccc(N2CCC3(CCCC3)CC2)cc1
[C:1]-[C:2]-[NH2;D1;+0:3]>>[C:1]-[C:2]-[NH;D2;+0:3]-[C:4](=[N;D1;H1:5])-[N;D1;H2:6]
null
[]
null
null
null
null
A solution of Example 287 (30 mg, 0.05 mmol), aminoiminosulfonic acid (7 mg, 0.055 mmol), diisopropylethylamine (0.02 M1), and DMF (0.3 mL) at room temperature was stirred for 24 hours and concentrated. The concentrate was purified by reverse phase chromatography with 0-90% methanol/0.1% aqueous TFA to provide the desi...
10.6084/m9.figshare.5104873.v1
null
Primary amine
Primary amine.Secondary amine
null
null
c1ccccc1.c1ccccc1.c1ccccc1.C1CCC2(C1)CC[NH]CC2
Other
null
null
null
NCCCC[C@H](CSc1ccccc1)Nc1ccc(S(=O)(=O)NC(=O)c2ccc(N3CCC4(CCCC4)CC3)cc2)cc1[N+](=O)[O-]>>N=C(N)NCCCC[C@H](CSc1ccccc1)Nc1ccc(S(=O)(=O)NC(=O)c2ccc(N3CCC4(CCCC4)CC3)cc2)cc1[N+](=O)[O-]
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a3e814fd460140f39cfae15c1ddd4afb
CCC(CC)(CO)CO.COC(=O)c1c(O)c(O)c(C(=O)OC)n1Cc1ccccc1>>CCC1(CC)COc2c(c(C(=O)OC)n(Cc3ccccc3)c2C(=O)OC)OC1
C(C)C(CO)(CO)CC.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.N(=NC(=O)OCC)C(=O)OCC.COC(=O)C=1N(C(=C(C1O)O)C(=O)OC)CC1=CC=CC=C1.N1C=CC=C1>>COC(=O)C=1N(C(=C2OCC(COC12)(CC)CC)C(=O)OC)CC1=CC=CC=C1
O[CH2:6][C:3]([CH2:2][CH3:1])([CH2:4][CH3:5])[CH2:29]O.[OH:7][c:8]1[c:9]([OH:28])[c:10]([C:11](=[O:12])[O:13][CH3:14])[n:15]([CH2:16][c:17]2[cH:18][cH:19][cH:20][cH:21][cH:22]2)[c:23]1[C:24](=[O:25])[O:26][CH3:27]>>[CH3:1][CH2:2][C:3]1([CH2:4][CH3:5])[CH2:6][O:7][c:8]2[c:9]([c:10]([C:11](=[O:12])[O:13][CH3:14])[n:15]([...
CCC(CC)(CO)CO.COC(=O)c1c(O)c(O)c(C(=O)OC)n1Cc1ccccc1
CCC1(CC)COc2c(c(C(=O)OC)n(Cc3ccccc3)c2C(=O)OC)OC1
null
null
O1CCCC1
Heteroatom Alkylation and Arylation
OtherReaction
1215c3f6aac7ca34fe457aa8add81c0a0f0dc07e98a78a57957222af48a54bc4
cd35ce5731247dee33d5ad312c41487245b509adde46d8f559cf867afeb9eba2
c1ccc(Cn2cc3c(c2)OCCCO3)cc1
O-[CH2;D2;+0:1]-[C:2](-[C:3])(-[C:4])-[CH2;D2;+0:5]-O.[#8:6]-[C:7](=[O;D1;H0:8])-[c:9]1:[#7;a:10](-[C:11]):[c:12](-[C:13](-[#8:14])=[O;D1;H0:15]):[c:16](-[OH;D1;+0:17]):[c:18]:1-[OH;D1;+0:19]>>[#8:6]-[C:7](=[O;D1;H0:8])-[c:9]1:[#7;a:10](-[C:11]):[c:12](-[C:13](-[#8:14])=[O;D1;H0:15]):[c:16]2:[c:18]:1-[O;H0;D2;+0:19]-[C...
null
[]
null
null
null
null
In the present method, 1-Benzyl-3,4-dihydroxy-1H-pyrrole-2,5-dicarboxylic acid dimethyl ester, the pyrrole derivative labeled A4 in FIG. 4 (hereinafter referred to as compound A4) is first synthesized from commercially available chemicals according to prior art techniques (see A. Merz, R. Schropp, E. Dotterl, “3,4-Dial...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Primary alcohol.Aromatic alcohol.Aromatic alcohol
Ether.Ether
null
C1COc2c[nH]cc2OC1
C1COc2c[nH]cc2OC1.c1ccccc1
HO-
O1CCCC1
null
null
CCC(CC)(CO)CO.COC(=O)c1c(O)c(O)c(C(=O)OC)n1Cc1ccccc1>O1CCCC1>CCC1(CC)COc2c(c(C(=O)OC)n(Cc3ccccc3)c2C(=O)OC)OC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4fcabc0faaaa4506ae4a26616316fe02
COC(=O)c1sc(C(=O)OC)c(O)c1O.C[Si]1(C)COc2cscc2OC1>>COC(=O)c1sc(C(=O)OC)c2c1OC[Si](C)(C)CO2
C[Si]1(COC2=CSC=C2OC1)C.COC(=O)C=1SC(=C(C1O)O)C(=O)OC.S1C=CC=C1.OC(O)[SiH](C)C.C1=CC=C(C=C1)P(C2=CC=CC=C2)C3=CC=CC=C3.CCOC(=O)/N=N/C(=O)OCC>>COC(=O)C=1SC(=C2OC[Si](COC12)(C)C)C(=O)OC
[CH3:1][O:2][C:3](=[O:4])[c:5]1[s:6][c:7]([C:8](=[O:9])[O:10][CH3:11])[c:12]([OH:20])[c:13]1[OH:14].c1scc2c1O[CH2:15][Si:16]([CH3:17])([CH3:18])[CH2:19]O2>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[s:6][c:7]([C:8](=[O:9])[O:10][CH3:11])[c:12]2[c:13]1[O:14][CH2:15][Si:16]([CH3:17])([CH3:18])[CH2:19][O:20]2
COC(=O)c1sc(C(=O)OC)c(O)c1O.C[Si]1(C)COc2cscc2OC1
COC(=O)c1sc(C(=O)OC)c2c1OC[Si](C)(C)CO2
null
null
O.C1CCOC1
Heteroatom Alkylation and Arylation
OtherReaction
7b6137ae600039f3bd8723aafc5c687f499e1388e832f227c897cac93b63c5f3
e37a086490c02521b04b2676ff92ea843071e75d56b8b4bb1a6a949554462337
c1scc2c1OC[SiH2]CO2
[#8:1]-[C:2](=[O;D1;H0:3])-[c:4]1:[#16;a:5]:[c:6](-[C:7](-[#8:8])=[O;D1;H0:9]):[c:10](-[OH;D1;+0:11]):[c:12]:1-[OH;D1;+0:13].[C;D1;H3:14]-[#14:15]1(-[C;D1;H3:16])-[CH2;D2;+0:17]-O-c2:c:s:c:c:2-O-[CH2;D2;+0:18]-1>>[#8:1]-[C:2](=[O;D1;H0:3])-[c:4]1:[#16;a:5]:[c:6](-[C:7](-[#8:8])=[O;D1;H0:9]):[c:10]2:[c:12]:1-[O;H0;D2;+0...
null
[]
null
null
null
null
A synthesis for 6,6-dimethyl-6,7-dihydro-5H-4,8-dioxa-2-thia-6-sila-azulene, a silicon-containing EC monomer generally related to 3,4-alkylenedioxythiophene, is shown in FIG. 7. First, 3,4-Dihydroxy-thiophene-2,5-dicarboxylic acid dimethyl ester, the thiophene derivative labeled A7 in FIG. 7 (hereinafter referred to as...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Aromatic alcohol.Aromatic alcohol
Ether.Ether
c1scc2c1OC[Si]CO2
c1scc2c1OC[Si]CO2
c1scc2c1OC[Si]CO2
Other
O.C1CCOC1
null
null
COC(=O)c1sc(C(=O)OC)c(O)c1O.C[Si]1(C)COc2cscc2OC1>O.C1CCOC1>COC(=O)c1sc(C(=O)OC)c2c1OC[Si](C)(C)CO2
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a3fb00f4f2f34bf4924744098467e41c
CC(=O)N1c2ccccc2[C@H](Nc2ccccc2)C[C@@H]1C.O=C(Cl)c1ccco1>>CC(=O)N1c2ccccc2[C@H](N(C(=O)c2ccco2)c2ccccc2)C[C@@H]1C
C[C@@H]1N(C2=CC=CC=C2[C@@H](C1)NC1=CC=CC=C1)C(C)=O.O1C(=CC=C1)C(=O)Cl.N1=CC=CC=C1>>C(C)(=O)N1[C@H](C[C@H](C2=CC=CC=C12)N(C(=O)C=1OC=CC1)C1=CC=CC=C1)C
[CH3:1][C:2](=[O:3])[N:4]1[c:5]2[cH:6][cH:7][cH:8][cH:9][c:10]2[C@H:11]([NH:12][c:20]2[cH:21][cH:22][cH:23][cH:24][cH:25]2)[CH2:26][C@@H:27]1[CH3:28].Cl[C:13](=[O:14])[c:15]1[cH:16][cH:17][cH:18][o:19]1>>[CH3:1][C:2](=[O:3])[N:4]1[c:5]2[cH:6][cH:7][cH:8][cH:9][c:10]2[C@H:11]([N:12]([C:13](=[O:14])[c:15]2[cH:16][cH:17][...
CC(=O)N1c2ccccc2[C@H](Nc2ccccc2)C[C@@H]1C.O=C(Cl)c1ccco1
CC(=O)N1c2ccccc2[C@H](N(C(=O)c2ccco2)c2ccccc2)C[C@@H]1C
null
null
C1(=CC=CC=C1)C
Acylation
N-alkylation of secondary amines with alkyl halides
b92e0bfd3d683c1f2a209adfe70a67ad7cb0d87749eb59e8fe0cf1689bc291e0
96cb0a2fed10552c5770a45a2d6523b47ac3e38928b4a9c698d8577451182dcd
O=C(c1ccco1)N(c1ccccc1)[C@@H]1CCNc2ccccc21
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6].[C:7]-[C:8](-[NH;D2;+0:9]-[c:10](:[c:11]):[c:12])-[c:13]>>[C:7]-[C:8](-[N;H0;D3;+0:9](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6])-[c:10](:[c:11]):[c:12])-[c:13]
40
[{"value": 40.0, "product": "C(C)(=O)N1[C@H](C[C@H](C2=CC=CC=C12)N(C(=O)C=1OC=CC1)C1=CC=CC=C1)C", "details": "PERCENTYIELD", "is_desired": false}]
90
CELSIUS
null
null
A round bottom flask under nitrogen atmosphere was charged with cis-(2-methyl-4-phenylamino-3,4-dihydro-2H-quinolin-1-yl)-ethanone (0.163 g, 0.58 mmol, 1.0 equiv) and 2-furoyl chloride (0.285 mL, 2.9 mmol, 5.0 equ), pyridine (1.0 equiv.) and dry toluene (3 mL). The solution was heated to 90° C. for 15 h. The reaction m...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Secondary amine
Tertiary amide
null
null
c1ccc2c(c1)CCC[NH]2.c1ccoc1.c1ccccc1
HCl
C1(=CC=CC=C1)C
90
null
CC(=O)N1c2ccccc2[C@H](Nc2ccccc2)C[C@@H]1C.O=C(Cl)c1ccco1>C1(=CC=CC=C1)C>CC(=O)N1c2ccccc2[C@H](N(C(=O)c2ccco2)c2ccccc2)C[C@@H]1C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7f925bc2320b4136acc246d65c313632
CC(=O)N1c2ccccc2[C@@H](Nc2ccccc2)C[C@@H]1C.O=C(Cl)c1ccco1>>CC(=O)N1c2ccccc2[C@@H](N(C(=O)c2ccco2)c2ccccc2)C[C@@H]1C
C[C@@H]1N(C2=CC=CC=C2[C@H](C1)NC1=CC=CC=C1)C(C)=O.O1C(=CC=C1)C(=O)Cl.N1=CC=CC=C1>>C(C)(=O)N1[C@H](C[C@@H](C2=CC=CC=C12)N(C(=O)C=1OC=CC1)C1=CC=CC=C1)C
[CH3:1][C:2](=[O:3])[N:4]1[c:5]2[cH:6][cH:7][cH:8][cH:9][c:10]2[C@@H:11]([NH:12][c:20]2[cH:21][cH:22][cH:23][cH:24][cH:25]2)[CH2:26][C@@H:27]1[CH3:28].Cl[C:13](=[O:14])[c:15]1[cH:16][cH:17][cH:18][o:19]1>>[CH3:1][C:2](=[O:3])[N:4]1[c:5]2[cH:6][cH:7][cH:8][cH:9][c:10]2[C@@H:11]([N:12]([C:13](=[O:14])[c:15]2[cH:16][cH:17...
CC(=O)N1c2ccccc2[C@@H](Nc2ccccc2)C[C@@H]1C.O=C(Cl)c1ccco1
CC(=O)N1c2ccccc2[C@@H](N(C(=O)c2ccco2)c2ccccc2)C[C@@H]1C
null
null
C1(=CC=CC=C1)C
Acylation
N-alkylation of secondary amines with alkyl halides
b92e0bfd3d683c1f2a209adfe70a67ad7cb0d87749eb59e8fe0cf1689bc291e0
96cb0a2fed10552c5770a45a2d6523b47ac3e38928b4a9c698d8577451182dcd
O=C(c1ccco1)N(c1ccccc1)[C@H]1CCNc2ccccc21
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6].[C:7]-[C:8](-[NH;D2;+0:9]-[c:10](:[c:11]):[c:12])-[c:13]>>[C:7]-[C:8](-[N;H0;D3;+0:9](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#8;a:5]:[c:6])-[c:10](:[c:11]):[c:12])-[c:13]
34
[{"value": 34.0, "product": "C(C)(=O)N1[C@H](C[C@@H](C2=CC=CC=C12)N(C(=O)C=1OC=CC1)C1=CC=CC=C1)C", "details": "PERCENTYIELD", "is_desired": false}]
50
CELSIUS
null
null
A round bottom flask under nitrogen atmosphere was charged with (±)-trans-1-(2-methyl-4-phenylamino-3,4-dihydro-2H-quinolin-1-yl)-ethanone (0.110 g, 0.39 mmol, 1.0 equiv) and 2-furoyl chloride (0.193 mL, 1.9 mmol, 5.0 equ), pyridine (1.0 equ.) and dry toluene (5 mL). The solution was heated to 50° C. for 5 h. The react...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Secondary amine
Tertiary amide
null
null
c1ccc2c(c1)CCC[NH]2.c1ccoc1.c1ccccc1
HCl
C1(=CC=CC=C1)C
50
null
CC(=O)N1c2ccccc2[C@@H](Nc2ccccc2)C[C@@H]1C.O=C(Cl)c1ccco1>C1(=CC=CC=C1)C>CC(=O)N1c2ccccc2[C@@H](N(C(=O)c2ccco2)c2ccccc2)C[C@@H]1C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8ce7c8db5ccf4775a9f4dd546229a7a7
CCN(C(C)C)C(C)C.C[C@H]1C[C@@H](Nc2ccccc2)c2ccccc2N1.O.O=C(Cl)c1ccco1>>CC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccco2)c2ccccc21
O.O1C(=CC=C1)C(=O)Cl.C[C@@H]1NC2=CC=CC=C2[C@@H](C1)NC1=CC=CC=C1.C(C)(C)N(CC)C(C)C>>O1C(=CC=C1)C(=O)N1[C@H](C[C@H](C2=CC=CC=C12)N(C(C)=O)C1=CC=CC=C1)C
CC(C)N(C(C)C)[CH2:2][CH3:1].[NH:4]([c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1)[C@@H:11]1[CH2:12][C@H:13]([CH3:14])[NH:15][c:23]2[cH:24][cH:25][cH:26][cH:27][c:28]21.[OH2:3].Cl[C:16](=[O:17])[c:18]1[cH:19][cH:20][cH:21][o:22]1>>[CH3:1][C:2](=[O:3])[N:4]([c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1)[C@@H:11]1[CH2:12][C@H:13]([CH3:...
CCN(C(C)C)C(C)C.C[C@H]1C[C@@H](Nc2ccccc2)c2ccccc2N1.O.O=C(Cl)c1ccco1
CC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccco2)c2ccccc21
null
null
ClCCl
Acylation
OtherReaction
d8fe791f0ca395497d722fb06b6ec821702194f4b653cb7bc63fa1b8371151dd
b1100398e30c6073eb2aa2e07cf07ab6770186d13e62a1cc70d851532cad5c0b
O=C(c1ccco1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
C-C(-C)-N(-[CH2;D2;+0:1]-[C;D1;H3:2])-C(-C)-C.Cl-[C;H0;D3;+0:3](=[O;D1;H0:4])-[c:5](:[c:6]):[#8;a:7]:[c:8].[C;D1;H3:9]-[C:10]1-[C:11]-[C:12](-[NH;D2;+0:13]-[c:14](:[c:15]):[c:16])-[c:17]:[c:18](:[c:19])-[NH;D2;+0:20]-1.[OH2;D0;+0:21]>>[C;D1;H3:9]-[C:10]1-[C:11]-[C:12](-[N;H0;D3;+0:13](-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;H...
83
[{"value": 83.0, "product": "O1C(=CC=C1)C(=O)N1[C@H](C[C@H](C2=CC=CC=C12)N(C(C)=O)C1=CC=CC=C1)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
12
HOUR
To a solution of (±)-cis-(2-Methyl-1,2,3,4-tetrahydro-quinolin-4-yl)-phenyl-amine (430 mg, 1.83 mmol) in dichloromethane (18 mL) at room temperature was added diisopropylethylamine (318 uL, 1.83 mmol) followed by 2-furoyl chloride. It was allowed to let stir at room temperature for 12 h. The mixture was poured into wat...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Secondary amine.Secondary amine.Tertiary amine
Tertiary amide.Tertiary amide
c1ccc2c(c1)CCCN2
c1ccc2c(c1)CCC[NH]2
c1ccccc1.c1ccoc1.c1ccc2c(c1)CCC[NH]2
HCl
ClCCl
null
12
CCN(C(C)C)C(C)C.C[C@H]1C[C@@H](Nc2ccccc2)c2ccccc2N1.O.O=C(Cl)c1ccco1>ClCCl>CC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccco2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1fb80b431d5b444e92a070f5b8a78d59
CC(=O)Cl.C[C@H]1C[C@@H](Nc2ccccc2)c2ccccc2N1C(=O)c1ccco1>>CC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccco2)c2ccccc21
O.C(C)(=O)Cl.O1C(=CC=C1)C(=O)N1[C@H](C[C@H](C2=CC=CC=C12)NC1=CC=CC=C1)C.C(C)(C)N(CC)C(C)C>>O1C(=CC=C1)C(=O)N1[C@H](C[C@H](C2=CC=CC=C12)N(C(C)=O)C1=CC=CC=C1)C
Cl[C:2]([CH3:1])=[O:3].[NH:4]([c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1)[C@@H:11]1[CH2:12][C@H:13]([CH3:14])[N:15]([C:16](=[O:17])[c:18]2[cH:19][cH:20][cH:21][o:22]2)[c:23]2[cH:24][cH:25][cH:26][cH:27][c:28]21>>[CH3:1][C:2](=[O:3])[N:4]([c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1)[C@@H:11]1[CH2:12][C@H:13]([CH3:14])[N:15]([C:1...
CC(=O)Cl.C[C@H]1C[C@@H](Nc2ccccc2)c2ccccc2N1C(=O)c1ccco1
CC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccco2)c2ccccc21
null
null
C(Cl)Cl
Acylation
N-alkylation of secondary amines with alkyl halides
b92e0bfd3d683c1f2a209adfe70a67ad7cb0d87749eb59e8fe0cf1689bc291e0
96cb0a2fed10552c5770a45a2d6523b47ac3e38928b4a9c698d8577451182dcd
O=C(c1ccco1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
Cl-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[C:4]-[C:5](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9])-[c:10]>>[C:4]-[C:5](-[N;H0;D3;+0:6](-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3])-[c:7](:[c:8]):[c:9])-[c:10]
61.4
[{"value": 57.0, "product": "O1C(=CC=C1)C(=O)N1[C@H](C[C@H](C2=CC=CC=C12)N(C(C)=O)C1=CC=CC=C1)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 61.4, "product": "O1C(=CC=C1)C(=O)N1[C@H](C[C@H](C2=CC=CC=C12)N(C(C)=O)C1=CC=CC=C1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of (±)-cis-furan-2-yl-(2-methyl-4-phenylamino-3,4-dihydro-2H-quinolin-1-yl)-methanone (360 mg, 1.0 mmol) in methylene chloride (5 mL) was added diisopropylethylamine (1.9 mL, 10 mmol) followed by acetyl chloride (388 uL, 5 mmol). The mixture was stirred at room temperature over night. The mixture was pour...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Secondary amine
Tertiary amide
null
null
c1ccccc1.c1ccoc1.c1ccc2c(c1)CCC[NH]2
HCl
C(Cl)Cl
null
null
CC(=O)Cl.C[C@H]1C[C@@H](Nc2ccccc2)c2ccccc2N1C(=O)c1ccco1>C(Cl)Cl>CC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccco2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2575977be9a34eada0d3c030887879c7
CC[C@H]1C[C@@H](N(C(C)=O)c2ccccc2)c2ccccc2N1C(=O)c1sc(-c2cnccn2)nc1C>>CC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2sc(-c3cnccn3)nc2C)c2ccccc21
C(C)[C@@H]1N(C2=CC=CC=C2[C@@H](C1)N(C(C)=O)C1=CC=CC=C1)C(=O)C1=C(N=C(S1)C1=NC=CN=C1)C.O1C(=CC=C1)C(=O)Cl>>C[C@@H]1N(C2=CC=CC=C2[C@@H](C1)N(C(C)=O)C1=CC=CC=C1)C(=O)C1=C(N=C(S1)C1=NC=CN=C1)C
C[CH2:14][C@H:13]1[CH2:12][C@@H:11]([N:4]([C:2]([CH3:1])=[O:3])[c:5]2[cH:6][cH:7][cH:8][cH:9][cH:10]2)[c:35]2[c:30]([cH:31][cH:32][cH:33][cH:34]2)[N:15]1[C:16](=[O:17])[c:18]1[s:19][c:20](-[c:21]2[cH:22][n:23][cH:24][cH:25][n:26]2)[n:27][c:28]1[CH3:29]>>[CH3:1][C:2](=[O:3])[N:4]([c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1)[...
CC[C@H]1C[C@@H](N(C(C)=O)c2ccccc2)c2ccccc2N1C(=O)c1sc(-c2cnccn2)nc1C
CC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2sc(-c3cnccn3)nc2C)c2ccccc21
null
null
null
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
O=C(c1cnc(-c2cnccn2)s1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
C-[CH2;D2;+0:1]-[C:2](-[C:3])-[#7:4](-[C:5]=[O;D1;H0:6])-[c:7]>>[C:3]-[C:2](-[CH3;D1;+0:1])-[#7:4](-[C:5]=[O;D1;H0:6])-[c:7]
null
[]
null
null
null
null
(±)-Cis-N-[2-ethyl-1-(4-methyl-2-pyrazin-2-yl-thiazole-5-carbonyl)-1,2,3,4-tetrahydro-quinolin-4-yl]-N-phenyl-acetamide was made following general procedure A, substituting 4-methyl-2-(2-pyrazinyl)-1,3-thiazole-5-carbonyl chloride for 2-furoyl chloride. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
c1ccccc1.c1cscn1.c1cnccn1.c1ccc2c(c1)CCC[NH]2
Other
null
null
null
CC[C@H]1C[C@@H](N(C(C)=O)c2ccccc2)c2ccccc2N1C(=O)c1sc(-c2cnccn2)nc1C>>CC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2sc(-c3cnccn3)nc2C)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d28d66c20b9943fc926c65ed8495c10c
CC1CC(N(C(=O)CO)c2ccccc2)c2ccccc2N1C(=O)c1ccc(F)cc1>>C[C@H]1C[C@@H](N(C(=O)CO)c2ccccc2)c2ccccc2N1C(=O)c1ccc(F)cc1
C(C)(=O)OCC(=O)Cl.FC1=CC=C(C(=O)N2C(CC(C3=CC=CC=C23)N(C(CO)=O)C2=CC=CC=C2)C)C=C1.FC1=CC=C(C(=O)Cl)C=C1.C(C)(=O)Cl.O1C(=CC=C1)C(=O)Cl>>FC1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N(C(CO)=O)C2=CC=CC=C2)C)C=C1
[CH3:1][CH:2]1[CH2:3][CH:4]([N:5]([C:6](=[O:7])[CH2:8][OH:9])[c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[N:22]1[C:23](=[O:24])[c:25]1[cH:26][cH:27][c:28]([F:29])[cH:30][cH:31]1>>[CH3:1][C@H:2]1[CH2:3][C@@H:4]([N:5]([C:6](=[O:7])[CH2:8][OH:9])[c:10]2[cH:11][cH:12][cH:13][cH:14]...
CC1CC(N(C(=O)CO)c2ccccc2)c2ccccc2N1C(=O)c1ccc(F)cc1
C[C@H]1C[C@@H](N(C(=O)CO)c2ccccc2)c2ccccc2N1C(=O)c1ccc(F)cc1
null
null
null
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
null
null
[]
null
null
null
null
(±)-N-[1-(4-fluoro-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-2-hydroxy-N-phenyl-acetamide was made following general procedure A substituting 4-fluorobenzoyl chloride for 2-furoyl chloride and acetoxyacetyl chloride for acetyl chloride. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
c1ccccc1.c1ccc2c(c1)CCC[NH]2.c1ccccc1
null
null
null
null
CC1CC(N(C(=O)CO)c2ccccc2)c2ccccc2N1C(=O)c1ccc(F)cc1>>C[C@H]1C[C@@H](N(C(=O)CO)c2ccccc2)c2ccccc2N1C(=O)c1ccc(F)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4e35c2b5ec1047f3870898d97fed7bac
CC[C@H]1C[C@@H](C(C)C(=O)Nc2ccccc2)c2ccccc2N1C(=O)c1cccnc1>>CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2cccnc2)c2ccccc21
C(CC)(=O)Cl.C(C)[C@@H]1N(C2=CC=CC=C2[C@@H](C1)C(C(=O)NC1=CC=CC=C1)C)C(=O)C=1C=NC=CC1.N1=CC(=CC=C1)Cl.C(C)(=O)Cl.O1C(=CC=C1)C(=O)Cl>>C[C@@H]1N(C2=CC=CC=C2[C@@H](C1)N(C(CC)=O)C1=CC=CC=C1)C(=O)C=1C=NC=CC1
C[CH2:15][C@H:14]1[CH2:13][C@@H:12]([CH:2]([CH3:1])[C:3](=[O:4])[NH:5][c:6]2[cH:7][cH:8][cH:9][cH:10][cH:11]2)[c:30]2[c:25]([cH:26][cH:27][cH:28][cH:29]2)[N:16]1[C:17](=[O:18])[c:19]1[cH:20][cH:21][cH:22][n:23][cH:24]1>>[CH3:1][CH2:2][C:3](=[O:4])[N:5]([c:6]1[cH:7][cH:8][cH:9][cH:10][cH:11]1)[C@@H:12]1[CH2:13][C@H:14](...
CC[C@H]1C[C@@H](C(C)C(=O)Nc2ccccc2)c2ccccc2N1C(=O)c1cccnc1
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2cccnc2)c2ccccc21
null
null
null
Miscellaneous
OtherReaction
32fece39de0f49f9e7ef15a495d62763f3f0bef4f24bac43aae52b9d127b312f
7fae2ddae661851fbaf2a59d877a8345033038358ec191ec2c5e2351a33f569b
O=C(c1cccnc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
C-[CH2;D2;+0:1]-[C:2]1-[C:3]-[C@@H;D3;+0:4](-[CH;D3;+0:5](-[C;D1;H3:6])-[C:7](=[O;D1;H0:8])-[NH;D2;+0:9]-[c:10](:[c:11]):[c:12])-[c:13](:[c:14]):[c:15]-[#7:16]-1-[C:17]=[O;D1;H0:18]>>[C;D1;H3:6]-[CH2;D2;+0:5]-[C:7](=[O;D1;H0:8])-[N;H0;D3;+0:9](-[C@@H;D3;+0:4]1-[C:3]-[C:2](-[CH3;D1;+0:1])-[#7:16](-[C:17]=[O;D1;H0:18])-[...
null
[]
null
null
null
null
(±)-Cis-[2-ethyl-1-(pyridine-3-carbonyl)-1,2,3,4-tetrahydro-quinolin-4-yl]-N-phenyl-propionamide was made following general procedure A substituting 3-pyridinyl chloride for 2-furoyl chloride and propionyl chloride for acetyl chloride. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Secondary amide
Tertiary amide
c1ccc2c(c1)CCC[NH]2
c1ccc2c(c1)CCC[NH]2
c1ccccc1.c1ccncc1.c1ccc2c(c1)CCC[NH]2
Other
null
null
null
CC[C@H]1C[C@@H](C(C)C(=O)Nc2ccccc2)c2ccccc2N1C(=O)c1cccnc1>>CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2cccnc2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-367a282312274d3c879236cf8fb82974
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(OC)c(F)c2)c2ccccc21.COc1ccc(C(=O)Cl)cc1F>>CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2cccc(OCF)c2)c2ccccc21
C(CC)(=O)Cl.FC=1C=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N(C(CC)=O)C2=CC=CC=C2)C)C=CC1OC.FC=1C=C(C(=O)Cl)C=CC1OC.C(C)(=O)Cl.O1C(=CC=C1)C(=O)Cl>>FCOC=1C=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N(C(CC)=O)C2=CC=CC=C2)C)C=CC1
CO[c:22]1[cH:21][cH:20][c:19]([C:17]([N:16]2[C@@H:14]([CH3:15])[CH2:13][C@@H:12]([N:5]([C:3]([CH2:2][CH3:1])=[O:4])[c:6]3[cH:7][cH:8][cH:9][cH:10][cH:11]3)[c:33]3[c:28]2[cH:29][cH:30][cH:31][cH:32]3)=[O:18])[cH:27][c:23]1F.C[O:24]c1ccc(C(=O)Cl)c[c:25]1[F:26]>>[CH3:1][CH2:2][C:3](=[O:4])[N:5]([c:6]1[cH:7][cH:8][cH:9][cH...
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(OC)c(F)c2)c2ccccc21.COc1ccc(C(=O)Cl)cc1F
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2cccc(OCF)c2)c2ccccc21
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
43b1f9bddc90103cd7ddd41a698fada63f32dc28dcbb28e997d1056d00d6eb4a
c9d3c1c0489a34084c35312557f2d1d020968105c809839f4243dffc35982739
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
C-O-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](-[C:5](-[#7:6])=[O;D1;H0:7]):[c:8]:[c;H0;D3;+0:9]:1-F.C-[O;H0;D2;+0:10]-c1:c:c:c(-C(-Cl)=O):c:[c;H0;D3;+0:11]:1-[F;D1;H0:12]>>[#7:6]-[C:5](=[O;D1;H0:7])-[c:4]1:[c:3]:[c:2]:[cH;D2;+0:1]:[c;H0;D3;+0:9](-[O;H0;D2;+0:10]-[CH2;D2;+0:11]-[F;D1;H0:12]):[c:8]:1
null
[]
null
null
null
null
(±)-Cis-N-[1-(3-fluoro-4-methoxy-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-N-phenyl-propionamide was made following general procedure A substituting 3-fluoro-4-methoxybenzoyl chloride for 2-furoyl chloride and propionyl chloride for acetyl chloride. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Aromatic halide.Aromatic halide.Ether.Ether
Primary halide.Ether
c1ccccc1.c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HF
null
null
null
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(OC)c(F)c2)c2ccccc21.COc1ccc(C(=O)Cl)cc1F>>CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2cccc(OCF)c2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-73fd8fecce2d48ac93c09fc0a7960966
CCOC(=O)N1CCC(c2ccc(C(=O)N3c4ccccc4[C@H](N(C(=O)CC)c4ccccc4)C[C@@H]3C)cc2)CC1>>CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(C3CCNCC3)cc2)c2ccccc21
C(C)OC(=O)N1CCC(CC1)C1=CC=C(C=C1)C(=O)N1[C@H](C[C@H](C2=CC=CC=C12)N(C(CC)=O)C1=CC=CC=C1)C.C(C)OC(=O)N1CCC(CC1)C1=CC=C(C=C1)C(=O)N1[C@H](C[C@H](C2=CC=CC=C12)N(C(CC)=O)C1=CC=CC=C1)C.I[Si](C)(C)C>>C[C@@H]1N(C2=CC=CC=C2[C@@H](C1)N(C(CC)=O)C1=CC=CC=C1)C(C1=CC=C(C=C1)C1CCNCC1)=O
CCOC(=O)[N:26]1[CH2:25][CH2:24][CH:23]([c:22]2[cH:21][cH:20][c:19]([C:17]([N:16]3[C@@H:14]([CH3:15])[CH2:13][C@@H:12]([N:5]([C:3]([CH2:2][CH3:1])=[O:4])[c:6]4[cH:7][cH:8][cH:9][cH:10][cH:11]4)[c:36]4[c:31]3[cH:32][cH:33][cH:34][cH:35]4)=[O:18])[cH:30][cH:29]2)[CH2:28][CH2:27]1>>[CH3:1][CH2:2][C:3](=[O:4])[N:5]([c:6]1[c...
CCOC(=O)N1CCC(c2ccc(C(=O)N3c4ccccc4[C@H](N(C(=O)CC)c4ccccc4)C[C@@H]3C)cc2)CC1
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(C3CCNCC3)cc2)c2ccccc21
null
null
C(C)#N
Reduction
Hydrogenolysis of tertiary amines
6dc5c07be2bf2a2ccc4ff166fd44281ea50e6dda805f74758334dcde1ad7a582
20c36f41eeb07c3ba4437b51ba72e8ff3c22d0b27e7197b0e9af3127f331149f
O=C(c1ccc(C2CCNCC2)cc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
C-C-O-C(=O)-[N;H0;D3;+0:1](-[C:2]-[C:3])-[C:4]-[C:5]>>[C:3]-[C:2]-[NH;D2;+0:1]-[C:4]-[C:5]
null
[]
null
null
null
null
(±)-Cis-N-[2-methyl-1-(4-piperidin-4-yl-benzoyl)-1,2,3,4-tetrahydro-quinolin-4-yl]-N-phenyl-propionamide was prepared from (±)-cis-4-{4-[2-methyl-4-(phenyl-propionyl-amino)-3,4-dihydro-2H-quinoline-1-carbonyl]-phenyl}-piperidine-1-carboxylic acid ethyl ester. (±)-Cis-4-{4-[2-methyl-4-(phenyl-propionyl-amino)-3,4-dihydr...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether
Secondary amine
C1CC[NH]CC1
C1CCNCC1
c1ccccc1.c1ccccc1.C1CCNCC1.c1ccc2c(c1)CCC[NH]2
HO-
C(C)#N
null
null
CCOC(=O)N1CCC(c2ccc(C(=O)N3c4ccccc4[C@H](N(C(=O)CC)c4ccccc4)C[C@@H]3C)cc2)CC1>C(C)#N>CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(C3CCNCC3)cc2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-827d3689fd1b434982c9c48ed847e029
CC(=O)Cl.NN1CCCCC1>>NC(=O)CN1CCCCC1
C([O-])(O)=O.[Na+].C(C)(C)N(CC)C(C)C.N1(CCCCC1)N.C(C)(=O)Cl>>N1(CCCCC1)CC(=O)N
Cl[C:2](=[O:3])[CH3:4].[NH2:1][N:5]1[CH2:6][CH2:7][CH2:8][CH2:9][CH2:10]1>>[NH2:1][C:2](=[O:3])[CH2:4][N:5]1[CH2:6][CH2:7][CH2:8][CH2:9][CH2:10]1
CC(=O)Cl.NN1CCCCC1
NC(=O)CN1CCCCC1
null
null
C(Cl)Cl
Acylation
OtherReaction
8b7d5514d87a925c0420829af26733388dfd75f01a0767d3fe8956f101d6629c
e5c25677803e61babaad51b064f83863eb4497268195d36f9f21f00b1069e47a
C1CCNCC1
Cl-[C;H0;D3;+0:1](-[CH3;D1;+0:2])=[O;D1;H0:3].[C:4]-[C:5]-[N;H0;D3;+0:6](-[NH2;D1;+0:7])-[C:8]-[C:9]>>[C:4]-[C:5]-[N;H0;D3;+0:6](-[CH2;D2;+0:2]-[C;H0;D3;+0:1](-[NH2;D1;+0:7])=[O;D1;H0:3])-[C:8]-[C:9]
100
[{"value": 100.0, "product": "N1(CCCCC1)CC(=O)N", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of the piperidine amine obtained above (676 mg, 1.59 mmol) in methylene chloride (25 mL) was added diisopropylethylamine (616 mg, 849 uL, 4.77 mmol), followed by acetyl chloride (162 mg, 156 uL, 2.06 mmol). The mixture was stirred at room temperature over night. The reaction mixture was poured into satura...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Hydrazine
Primary amide.Tertiary amine
C1CC[NH]CC1
C1CC[NH]CC1
C1CC[NH]CC1
HCl
C(Cl)Cl
null
null
CC(=O)Cl.NN1CCCCC1>C(Cl)Cl>NC(=O)CN1CCCCC1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-74cf2a8ed51c46379e5143067e800f17
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc([N+](=O)[O-])cc2)c2ccccc21>>CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N)cc2)c2ccccc21
C[C@@H]1N(C2=CC=CC=C2[C@@H](C1)N(C(CC)=O)C1=CC=CC=C1)C(C1=CC=C(C=C1)[N+](=O)[O-])=O>>NC1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N(C(CC)=O)C2=CC=CC=C2)C)C=C1
O=[N+:23]([O-])[c:22]1[cH:21][cH:20][c:19]([C:17]([N:16]2[C@@H:14]([CH3:15])[CH2:13][C@@H:12]([N:5]([C:3]([CH2:2][CH3:1])=[O:4])[c:6]3[cH:7][cH:8][cH:9][cH:10][cH:11]3)[c:31]3[c:26]2[cH:27][cH:28][cH:29][cH:30]3)=[O:18])[cH:25][cH:24]1>>[CH3:1][CH2:2][C:3](=[O:4])[N:5]([c:6]1[cH:7][cH:8][cH:9][cH:10][cH:11]1)[C@@H:12]1...
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc([N+](=O)[O-])cc2)c2ccccc21
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N)cc2)c2ccccc21
null
[Pd]
C(C)O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
86
[{"value": 86.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
(±)-Cis-N-[1-(4-amino-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-N-phenyl-propionamide was prepared from (±)-cis-N-[2-methylmethyl-1-(4-nitro-benzoyl)-1,2,3,4-tetrahydro-quinolin-4-yl]-N-phenyl-propionamide. (±)-Cis-N-[2-methyl-1-(4-nitro-benzoyl)-1,2,3,4-tetrahydro-quinolin-4-yl]-N-phenyl-propionamide (200 mg...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
Other
[Pd].C(C)O
null
null
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc([N+](=O)[O-])cc2)c2ccccc21>[Pd].C(C)O>CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N)cc2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8829c1768c024d90ac6b20c3195368cf
CC(=O)Cl.CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N)cc2)c2ccccc21>>CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(NC(C)=O)cc2)c2ccccc21
C(C)N(CC)CC.NC1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N(C(CC)=O)C2=CC=CC=C2)C)C=C1.NC1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N(C(CC)=O)C2=CC=CC=C2)C)C=C1.C(C)(=O)Cl>>C(C)(=O)NC1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N(C(CC)=O)C2=CC=CC=C2)C)C=C1
Cl[C:24]([CH3:25])=[O:26].[CH3:1][CH2:2][C:3](=[O:4])[N:5]([c:6]1[cH:7][cH:8][cH:9][cH:10][cH:11]1)[C@@H:12]1[CH2:13][C@H:14]([CH3:15])[N:16]([C:17](=[O:18])[c:19]2[cH:20][cH:21][c:22]([NH2:23])[cH:27][cH:28]2)[c:29]2[cH:30][cH:31][cH:32][cH:33][c:34]21>>[CH3:1][CH2:2][C:3](=[O:4])[N:5]([c:6]1[cH:7][cH:8][cH:9][cH:10][...
CC(=O)Cl.CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N)cc2)c2ccccc21
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(NC(C)=O)cc2)c2ccccc21
null
null
O1CCCC1
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
Cl-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[NH2;D1;+0:4]-[c:5](:[c:6]):[c:7]>>[C;D1;H3:2]-[C;H0;D3;+0:1](=[O;D1;H0:3])-[NH;D2;+0:4]-[c:5](:[c:6]):[c:7]
46
[{"value": 46.0, "product": "C(C)(=O)NC1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N(C(CC)=O)C2=CC=CC=C2)C)C=C1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
(±)-Cis-N-[1-(4-acetylamino-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-N-phenyl-propionamide was prepared from (±)-cis-N-[1-(4-amino-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-N-phenyl-propionamide. To a solution of (±)-cis-N-[1-(4-amino-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-N-phenyl-pro...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HCl
O1CCCC1
null
8
CC(=O)Cl.CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N)cc2)c2ccccc21>O1CCCC1>CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(NC(C)=O)cc2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-afd5bdb5e9ec4016b8f7918cf852fbd9
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N)cc2)c2ccccc21.CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N)cc2)c2ccccc21.CCC(=O)O>>CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(-n3c(C)ccc3C)cc2)c2ccccc21
NC1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N(C(CC)=O)C2=CC=CC=C2)C)C=C1.NC1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N(C(CC)=O)C2=CC=CC=C2)C)C=C1.C(CC)(=O)O.C1=CC=CC=C1>>CC=1N(C(=CC1)C)C1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N(C(CC)=O)C2=CC=CC=C2)C)C=C1
[CH3:1][CH2:2][C:3](=[O:4])[N:5]([c:6]1[cH:7][cH:8][cH:9][cH:10][cH:11]1)[C@@H:12]1[CH2:13][C@H:14]([CH3:15])[N:16]([C:17](=[O:18])[c:19]2[cH:20][cH:21][c:22]([NH2:23])[cH:30][cH:31]2)[c:32]2[cH:33][cH:34][cH:35][cH:36][c:37]21.Nc1ccc(C(=O)N2c3ccccc3[C@H](N(C(=O)[CH2:28][CH3:29])c3ccccc3)C[C@@H]2[CH3:25])cc1.O=[C:24](O...
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N)cc2)c2ccccc21.CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N)cc2)c2ccccc21.CCC(=O)O
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(-n3c(C)ccc3C)cc2)c2ccccc21
null
null
null
C-C Coupling
OtherReaction
16a13f13bd674386af51fe2e696231ee34c5fd93d09332408df064455b84a965
b0c8191f272b36b270edc62d5fbc09fbff0891556a7d8513b38018083a26d939
O=C(c1ccc(-n2cccc2)cc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
N-c1:c:c:c(-C(=O)-N2-[C@H](-[CH3;D1;+0:1])-C-[C@H](-N(-C(=O)-[CH2;D2;+0:2]-[C;D1;H3:3])-c3:c:c:c:c:c:3)-c3:c:c:c:c:c:3-2):c:c:1.O-[C;H0;D3;+0:4](=O)-[CH2;D2;+0:5]-[CH3;D1;+0:6].[NH2;D1;+0:7]-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[C;D1;H3:3]-[c;H0;D3;+0:2]1:[cH;D2;+0:6]:[cH;D2;+0:5]:[c;H0;D3;+0:4](-[CH3;D1;+0:1])...
80
[{"value": 80.0, "product": "CC=1N(C(=CC1)C)C1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N(C(CC)=O)C2=CC=CC=C2)C)C=C1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
(±)-Cis-N-{1-[4-(2,5-dimethyl-pyrrol-1-yl)-benzoyl]-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl}-N-phenyl-propionamide was prepared from (±)-cis-N-[1-(4-amino-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-N-phenyl-propionamide. A solution of (±)-cis-N-[1-(4-amino-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Tertiary amide.Tertiary amide.Primary amine.Primary amine
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCCN2
c1ccc[nH]1
c1ccccc1.c1ccccc1.c1ccc[nH]1.c1ccc2c(c1)CCC[NH]2
HO-
null
null
null
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N)cc2)c2ccccc21.CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N)cc2)c2ccccc21.CCC(=O)O>>CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(-n3c(C)ccc3C)cc2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b6c2f061c4224b129271530af5a78add
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N)cc2)c2ccccc21.CCC(C=O)CC>>CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(NCC(CC)CC)cc2)c2ccccc21
C(C)(=O)O[BH-](OC(C)=O)OC(C)=O.[Na+].NC1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N(C(CC)=O)C2=CC=CC=C2)C)C=C1.C(C)C(C=O)CC.NC1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N(C(CC)=O)C2=CC=CC=C2)C)C=C1.C(C)(=O)O>>C(C)C(CNC1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N(C(CC)=O)C2=CC=CC=C2)C)C=C1)CC
[CH3:1][CH2:2][C:3](=[O:4])[N:5]([c:6]1[cH:7][cH:8][cH:9][cH:10][cH:11]1)[C@@H:12]1[CH2:13][C@H:14]([CH3:15])[N:16]([C:17](=[O:18])[c:19]2[cH:20][cH:21][c:22]([NH2:23])[cH:30][cH:31]2)[c:32]2[cH:33][cH:34][cH:35][cH:36][c:37]21.O=[CH:24][CH:25]([CH2:26][CH3:27])[CH2:28][CH3:29]>>[CH3:1][CH2:2][C:3](=[O:4])[N:5]([c:6]1[...
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N)cc2)c2ccccc21.CCC(C=O)CC
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(NCC(CC)CC)cc2)c2ccccc21
null
null
ClCCl
Heteroatom Alkylation and Arylation
Reductive amination with aldehyde
422be648aea52bce28ccc8fb32ec3178aaa47bbd624f063874619362f075b5f2
7915721a3e395aed85e3c40dc4d725c571a931ac517c6a0da16f2a2b0bb5eac7
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
O=[CH;D2;+0:1]-[C:2](-[C:3])-[C:4].[NH2;D1;+0:5]-[c:6](:[c:7]):[c:8]>>[C:3]-[C:2](-[C:4])-[CH2;D2;+0:1]-[NH;D2;+0:5]-[c:6](:[c:7]):[c:8]
83
[{"value": 83.0, "product": "C(C)C(CNC1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N(C(CC)=O)C2=CC=CC=C2)C)C=C1)CC", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
(±)-Cis-N-{1-[4-(2-ethyl-butylamino)-benzoyl]-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl}-N-phenyl-propionamide was prepared from (±)-cis-N-[1-(4-amino-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-N-phenyl-propionamide. To a solution of (±)-cis-N-[1-(4-Amino-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-N-p...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary amine
Secondary amine
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
Other
ClCCl
null
null
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N)cc2)c2ccccc21.CCC(C=O)CC>ClCCl>CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(NCC(CC)CC)cc2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-290a98cf79694152b7a09c981c128001
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N)cc2)c2ccccc21.CCC=O>>CCCNc1ccc(C(=O)N2c3ccccc3[C@H](N(C(=O)CC)c3ccccc3)C[C@@H]2C)cc1
C(C)C(C=O)CC.C(C)C(CNC1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N(C(CC)=O)C2=CC=CC=C2)C)C=C1)CC.NC1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N(C(CC)=O)C2=CC=CC=C2)C)C=C1.C(CC)=O>>C[C@@H]1N(C2=CC=CC=C2[C@@H](C1)N(C(CC)=O)C1=CC=CC=C1)C(C1=CC=C(C=C1)NCCC)=O
[NH2:4][c:5]1[cH:6][cH:7][c:8]([C:9](=[O:10])[N:11]2[c:12]3[cH:13][cH:14][cH:15][cH:16][c:17]3[C@H:18]([N:19]([C:20](=[O:21])[CH2:22][CH3:23])[c:24]3[cH:25][cH:26][cH:27][cH:28][cH:29]3)[CH2:30][C@@H:31]2[CH3:32])[cH:33][cH:34]1.O=[CH:3][CH2:2][CH3:1]>>[CH3:1][CH2:2][CH2:3][NH:4][c:5]1[cH:6][cH:7][c:8]([C:9](=[O:10])[N...
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N)cc2)c2ccccc21.CCC=O
CCCNc1ccc(C(=O)N2c3ccccc3[C@H](N(C(=O)CC)c3ccccc3)C[C@@H]2C)cc1
null
null
null
Heteroatom Alkylation and Arylation
Reductive amination with aldehyde
422be648aea52bce28ccc8fb32ec3178aaa47bbd624f063874619362f075b5f2
7915721a3e395aed85e3c40dc4d725c571a931ac517c6a0da16f2a2b0bb5eac7
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
O=[CH;D2;+0:1]-[C:2]-[C;D1;H3:3].[NH2;D1;+0:4]-[c:5](:[c:6]):[c:7]>>[C;D1;H3:3]-[C:2]-[CH2;D2;+0:1]-[NH;D2;+0:4]-[c:5](:[c:6]):[c:7]
null
[]
null
null
null
null
(±)-Cis-N-[2-methyl-1-(4-propylamino-benzoyl)-1,2,3,4-tetrahydro-quinolin-4-yl]-N-phenyl-propionamide was prepared from (±)-cis-N-[1-(4-amino-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-N-phenyl-propionamide utilizing the reductive amination conditions described for the synthesis of (±)-cis-N-{1-[4-(2-ethyl-but...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary amine
Secondary amine
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
Other
null
null
null
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N)cc2)c2ccccc21.CCC=O>>CCCNc1ccc(C(=O)N2c3ccccc3[C@H](N(C(=O)CC)c3ccccc3)C[C@@H]2C)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4ac644dd7a2141dea55bcae060251f8c
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N)cc2)c2ccccc21.COC(=O)C(C)Br>>COC(=O)C(C)Nc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccccc3)C[C@@H]2C)cc1
NC1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N(C(CC)=O)C2=CC=CC=C2)C)C=C1.NC1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N(C(CC)=O)C2=CC=CC=C2)C)C=C1.C([O-])([O-])=O.[K+].[K+].BrC(C(=O)OC)C.O>>COC(C(C)NC1=CC=C(C=C1)C(=O)N1[C@H](C[C@H](C2=CC=CC=C12)N(C1=CC=CC=C1)C(C)=O)C)=O
C[CH2:24][C:23]([N:22]([C@H:21]1[c:20]2[c:15]([cH:16][cH:17][cH:18][cH:19]2)[N:14]([C:12]([c:11]2[cH:10][cH:9][c:8]([NH2:7])[cH:36][cH:35]2)=[O:13])[C@@H:33]([CH3:34])[CH2:32]1)[c:26]1[cH:27][cH:28][cH:29][cH:30][cH:31]1)=[O:25].Br[CH:5]([C:3]([O:2][CH3:1])=[O:4])[CH3:6]>>[CH3:1][O:2][C:3](=[O:4])[CH:5]([CH3:6])[NH:7][...
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N)cc2)c2ccccc21.COC(=O)C(C)Br
COC(=O)C(C)Nc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccccc3)C[C@@H]2C)cc1
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
OtherReaction
9460f8aba9fd9df7be6d8646a415233de3960f11da8401461639ab4fc047b682
ce839c3e1095e851f2e0a7549fc2029a1d2ad47a8a3c3a46b00a63b754bc5ab7
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
Br-[CH;D3;+0:1](-[C;D1;H3:2])-[C:3](=[O;D1;H0:4])-[#8:5]-[C;D1;H3:6].C-[CH2;D2;+0:7]-[C:8](=[O;D1;H0:9])-[#7:10](-[C:11])-[c:12].[NH2;D1;+0:13]-[c:14](:[c:15]):[c:16]>>[C;D1;H3:6]-[#8:5]-[C:3](=[O;D1;H0:4])-[CH;D3;+0:1](-[C;D1;H3:2])-[NH;D2;+0:13]-[c:14](:[c:15]):[c:16].[C:11]-[#7:10](-[c:12])-[C:8](-[CH3;D1;+0:7])=[O;...
87
[{"value": 87.0, "product": "COC(C(C)NC1=CC=C(C=C1)C(=O)N1[C@H](C[C@H](C2=CC=CC=C12)N(C1=CC=CC=C1)C(C)=O)C)=O", "details": "PERCENTYIELD", "is_desired": false}]
100
CELSIUS
null
null
(±)-Cis-2-{4-[4-(acetyl-phenyl-amino)-2-methyl-3,4-dihydro-2H-quinoline-1-carbonyl]-phenylamino}-propionic acid methyl ester was prepared from (±)-cis-N-[1-(4-amino-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-N-phenyl-propionamide. A mixture of (±)-cis-N-[1-(4-amino-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin...
10.6084/m9.figshare.5104873.v1
null
Secondary halide.Ester.Primary amine
Ester.Secondary amine
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HBr
CN(C=O)C
100
null
CCC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N)cc2)c2ccccc21.COC(=O)C(C)Br>CN(C=O)C>COC(=O)C(C)Nc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccccc3)C[C@@H]2C)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d0d62d144b904d71baaab5ea2a058acc
COc1cccc(CBr)c1.C[C@H]1C[C@@H](Nc2ccccc2)c2ccccc2N1>>COc1cccc(CN2c3ccccc3[C@H](N(C(C)=O)c3ccccc3)C[C@@H]2C)c1
C([O-])([O-])=O.[K+].[K+].C[C@@H]1NC2=CC=CC=C2[C@@H](C1)NC1=CC=CC=C1.CN(C=O)C.BrCC1=CC(=CC=C1)OC.[I-].[K+]>>COC=1C=C(CN2[C@H](C[C@H](C3=CC=CC=C23)N(C(C)=O)C2=CC=CC=C2)C)C=CC1
Br[CH2:8][c:7]1[cH:6][cH:5][cH:4][c:3]([O:2][CH3:1])[cH:30]1.[NH:9]1[c:10]2[cH:11][cH:12][cH:13][cH:14][c:15]2[C@H:16]([NH:17][c:21]2[cH:22][cH:23][cH:24][cH:25][cH:26]2)[CH2:27][C@@H:28]1[CH3:29]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7]([CH2:8][N:9]2[c:10]3[cH:11][cH:12][cH:13][cH:14][c:15]3[C@H:16]([N:17]([C:18]([C...
COc1cccc(CBr)c1.C[C@H]1C[C@@H](Nc2ccccc2)c2ccccc2N1
COc1cccc(CN2c3ccccc3[C@H](N(C(C)=O)c3ccccc3)C[C@@H]2C)c1
null
null
null
Acylation
OtherReaction
89ca2ffbea3ec23ad760d7d7bda55bf4f95e7326c1643fb731ace5c8f5519feb
8edf1c26d504354a50dce45786b72c1940be701838dd8c41b265bdb7308b60c1
c1ccc(CN2CC[C@@H](Nc3ccccc3)c3ccccc32)cc1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[C;D1;H3:5]-[C:6]1-[C:7]-[C:8](-[NH;D2;+0:9]-[c:10](:[c:11]):[c:12])-[c:13]:[c:14](:[c:15])-[NH;D2;+0:16]-1>>[C;D1;H3:17]-[C:18](=[O;D1;H0:19])-[N;H0;D3;+0:9](-[C:8]1-[C:7]-[C:6](-[C;D1;H3:5])-[N;H0;D3;+0:16](-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4])-[c:14](:[c:15]):[c:13]-1)-[c:10](:[c:1...
null
[]
null
null
null
null
(±)-Cis-N-[1-(3-methoxy-benzyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-N-phenyl-acetamide was synthesized by dissolving (±)-cis-(2-methyl-1,2,3,4-tetrahydroquinol-4-yl)aniline in dimethylformamide and adding potassium carbonate (1.0-10.0 equiv.), and the 1-bromomethyl-3-methoxy-benzene (1.1-3.0 equiv), catalytic po...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amine.Secondary amine
Tertiary amide.Tertiary amine
c1ccc2c(c1)CCCN2
c1ccc2c(c1)CCC[NH]2
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
Br-
null
null
null
COc1cccc(CBr)c1.C[C@H]1C[C@@H](Nc2ccccc2)c2ccccc2N1>>COc1cccc(CN2c3ccccc3[C@H](N(C(C)=O)c3ccccc3)C[C@@H]2C)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c31dcfe8f0c146db87d63e5e85a21e53
CCN=C=O.COc1cccc(C(=O)N2c3ccccc3[C@H](Nc3ccccc3)C[C@@H]2C)c1>>CCNC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2cccc(OC)c2)c2ccccc21
C(C)(=O)Cl.COC=1C=C(C=CC1)C(=O)N1[C@H](C[C@H](C2=CC=CC=C12)NC1=CC=CC=C1)C.C(C)N=C=O>>C(C)NC(N(C1=CC=CC=C1)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC(=CC=C1)OC)=O)C)=O
[CH3:1][CH2:2][N:3]=[C:4]=[O:5].[NH:6]([c:7]1[cH:8][cH:9][cH:10][cH:11][cH:12]1)[C@@H:13]1[CH2:14][C@H:15]([CH3:16])[N:17]([C:18](=[O:19])[c:20]2[cH:21][cH:22][cH:23][c:24]([O:25][CH3:26])[cH:27]2)[c:28]2[cH:29][cH:30][cH:31][cH:32][c:33]21>>[CH3:1][CH2:2][NH:3][C:4](=[O:5])[N:6]([c:7]1[cH:8][cH:9][cH:10][cH:11][cH:12]...
CCN=C=O.COc1cccc(C(=O)N2c3ccccc3[C@H](Nc3ccccc3)C[C@@H]2C)c1
CCNC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2cccc(OC)c2)c2ccccc21
null
null
CN(C)C=O
Acylation
Urea synthesis via isocyanate and secondary amine
288f31369c46060b9009e57afc96d52a76d6a0243a2e1197ab47b0221bb8a3ee
5272a383a93723269f1934f97993b0175b43cd993bcdf2f45add1dbb852d1e09
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
[C;D1;H3:1]-[C:2]-[N;H0;D2;+0:3]=[C;H0;D2;+0:4]=[O;D1;H0:5].[C:6]-[C:7](-[NH;D2;+0:8]-[c:9](:[c:10]):[c:11])-[c:12]>>[C:6]-[C:7](-[N;H0;D3;+0:8](-[C;H0;D3;+0:4](=[O;D1;H0:5])-[NH;D2;+0:3]-[C:2]-[C;D1;H3:1])-[c:9](:[c:10]):[c:11])-[c:12]
null
[]
90
CELSIUS
null
null
(±)-Cis-3-ethyl-1-[1-(3-methoxy-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-1-phenyl-urea was synthesized using general procedure A, substituting ethyl isocyanate for acetyl chloride using the following procedure. To a solution of (±)-cis-(3-methoxy-phenyl)-(2-methyl-4-anilino-3,4-dihydro-2H-quinolin-1-yl)-meth...
10.6084/m9.figshare.5104873.v1
null
Isocyanate.Secondary amine
Urea
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
null
CN(C)C=O
90
null
CCN=C=O.COc1cccc(C(=O)N2c3ccccc3[C@H](Nc3ccccc3)C[C@@H]2C)c1>CN(C)C=O>CCNC(=O)N(c1ccccc1)[C@@H]1C[C@H](C)N(C(=O)c2cccc(OC)c2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-06f6d363cb3f4d8fbdd4a0ddadbf7f8f
C=CNC(=O)OCc1ccccc1.CC=O.Nc1ccccc1>>C[C@H]1C[C@@H](NC(=O)OCc2ccccc2)c2ccccc2N1
C(C1=CC=CC=C1)OC(NC=C)=O.NC1=CC=CC=C1.[O-]S(=O)(=O)[O-].[Na+].[Na+].B(F)(F)F.CCOCC.C(C)=O>>C(C1=CC=CC=C1)OC(N[C@@H]1C[C@@H](NC2=CC=CC=C12)C)=O
[CH2:3]=[CH:4][NH:5][C:6](=[O:7])[O:8][CH2:9][c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1.O=[CH:2][CH3:1].[cH:16]1[cH:17][cH:18][cH:19][cH:20][c:21]1[NH2:22]>>[CH3:1][C@H:2]1[CH2:3][C@@H:4]([NH:5][C:6](=[O:7])[O:8][CH2:9][c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[NH:22]1
C=CNC(=O)OCc1ccccc1.CC=O.Nc1ccccc1
C[C@H]1C[C@@H](NC(=O)OCc2ccccc2)c2ccccc2N1
null
null
C(Cl)Cl
Heteroatom Alkylation and Arylation
OtherReaction
10a367808e4d8a02f921e4f22ccec96cb0760c79632f6e1bfbd759fd1bea15ff
afc6fb3b06bcafaed087853b7812fac61e988e823b4d4d1a5152296d73d10689
O=C(N[C@@H]1CCNc2ccccc21)OCc1ccccc1
O=[CH;D2;+0:1]-[C;D1;H3:2].[#8:3]-[C:4](=[O;D1;H0:5])-[#7:6]-[CH;D2;+0:7]=[CH2;D1;+0:8].[NH2;D1;+0:9]-[c:10](:[c:11]):[cH;D2;+0:12]:[c:13]:[c:14]>>[#8:3]-[C:4](=[O;D1;H0:5])-[#7:6]-[C@@H;D3;+0:7]1-[CH2;D2;+0:8]-[C@H;D3;+0:1](-[C;D1;H3:2])-[NH;D2;+0:9]-[c:10](:[c:11]):[c;H0;D3;+0:12]-1:[c:13]:[c:14]
33.8
[{"value": 33.0, "product": "C(C1=CC=CC=C1)OC(N[C@@H]1C[C@@H](NC2=CC=CC=C12)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 33.8, "product": "C(C1=CC=CC=C1)OC(N[C@@H]1C[C@@H](NC2=CC=CC=C12)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-25
CELSIUS
1
HOUR
Aniline (3.64 mL, 39.97 mmol, 1.0 equ) was dissolved in methylene chloride (100 mL) and Na2SO4 (2 g) was added and cooled to −25° C. Acetaldehyde (2.23 mL, 39.97 mmol, 1.0 equ.) was added to the solution and stirred for 1 h at −25° C. Sodium sulfate was filtered off and N-vinyl-carbamic acid benzyl ester (7.07 g, 39.97...
10.6084/m9.figshare.5104873.v1
null
Enamine.Aldehyde.Primary amine
Secondary amine
c1ccccc1
c1ccc2c(c1)CCCN2
c1ccccc1.c1ccc2c(c1)CCCN2
HO-
C(Cl)Cl
-25
1
C=CNC(=O)OCc1ccccc1.CC=O.Nc1ccccc1>C(Cl)Cl>C[C@H]1C[C@@H](NC(=O)OCc2ccccc2)c2ccccc2N1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-cd63f102ed484888810a8935670de1da
CN(C)c1ccc(C(=O)Cl)cc1.C[C@H]1C[C@@H](NC(=O)OCc2ccccc2)c2ccccc2N1>>C[C@H]1C[C@@H](NC(=O)OCc2ccccc2)c2ccccc2N1C(=O)c1ccc(N(C)C)cc1
O.CN(C1=CC=C(C(=O)Cl)C=C1)C.C(C1=CC=CC=C1)OC(N[C@@H]1C[C@@H](NC2=CC=CC=C12)C)=O.C(C)(C)N(CC)C(C)C>>C(C1=CC=CC=C1)OC(N[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)N(C)C)=O)C)=O
Cl[C:23](=[O:24])[c:25]1[cH:26][cH:27][c:28]([N:29]([CH3:30])[CH3:31])[cH:32][cH:33]1.[CH3:1][C@H:2]1[CH2:3][C@@H:4]([NH:5][C:6](=[O:7])[O:8][CH2:9][c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[NH:22]1>>[CH3:1][C@H:2]1[CH2:3][C@@H:4]([NH:5][C:6](=[O:7])[O:8][CH2:9][c:10]2[cH:11]...
CN(C)c1ccc(C(=O)Cl)cc1.C[C@H]1C[C@@H](NC(=O)OCc2ccccc2)c2ccccc2N1
C[C@H]1C[C@@H](NC(=O)OCc2ccccc2)c2ccccc2N1C(=O)c1ccc(N(C)C)cc1
null
null
C(Cl)Cl
Acylation
N-alkylation of secondary amines with alkyl halides
20af49e2ebd8e13ce8273786fd70e980d9c80eb9362be37fe2fe9cf2d75c9b8d
96cb0a2fed10552c5770a45a2d6523b47ac3e38928b4a9c698d8577451182dcd
O=C(N[C@@H]1CCN(C(=O)c2ccccc2)c2ccccc21)OCc1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C:6]-[C:7](-[C;D1;H3:8])-[NH;D2;+0:9]-[c:10](:[c:11]):[c:12]>>[C:6]-[C:7](-[C;D1;H3:8])-[N;H0;D3;+0:9](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5])-[c:10](:[c:11]):[c:12]
89
[{"value": 89.0, "product": "C(C1=CC=CC=C1)OC(N[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)N(C)C)=O)C)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of (±)-cis-(2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl)-carbamic acid benzyl ester (500 mg, 1.68 mmol) in methylene chloride (20 mL) at room temperature was added diisopropylethylamine (542 mg, 749 uL, 4.2 mmol) followed by 4-dimethylaminobenzoyl chloride and stirred at room temperature until no starting m...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Secondary amine
Tertiary amide
c1ccc2c(c1)CCCN2
c1ccc2c(c1)CCC[NH]2
c1ccccc1.c1ccc2c(c1)CCC[NH]2.c1ccccc1
HCl
C(Cl)Cl
null
null
CN(C)c1ccc(C(=O)Cl)cc1.C[C@H]1C[C@@H](NC(=O)OCc2ccccc2)c2ccccc2N1>C(Cl)Cl>C[C@H]1C[C@@H](NC(=O)OCc2ccccc2)c2ccccc2N1C(=O)c1ccc(N(C)C)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4e4a6aa273e64d5ea72cc4632fb25e8e
C[C@H]1C[C@@H](NC(=O)OCc2ccccc2)c2ccccc2N1C(=O)c1ccc(N(C)C)cc1>>C[C@H]1C[C@@H](N)c2ccccc2N1C(=O)c1ccc(N(C)C)cc1
C(C1=CC=CC=C1)OC(N[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)N(C)C)=O)C)=O>>CN(C1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N)C)C=C1)C
O=C(OCc1ccccc1)[NH:5][C@@H:4]1[CH2:3][C@H:2]([CH3:1])[N:12]([C:13](=[O:14])[c:15]2[cH:16][cH:17][c:18]([N:19]([CH3:20])[CH3:21])[cH:22][cH:23]2)[c:11]2[c:6]1[cH:7][cH:8][cH:9][cH:10]2>>[CH3:1][C@H:2]1[CH2:3][C@@H:4]([NH2:5])[c:6]2[cH:7][cH:8][cH:9][cH:10][c:11]2[N:12]1[C:13](=[O:14])[c:15]1[cH:16][cH:17][c:18]([N:19]([...
C[C@H]1C[C@@H](NC(=O)OCc2ccccc2)c2ccccc2N1C(=O)c1ccc(N(C)C)cc1
C[C@H]1C[C@@H](N)c2ccccc2N1C(=O)c1ccc(N(C)C)cc1
null
null
C(C)O
Reduction
Hydrogenolysis of amides/imides/carbamates
087b6600ba91d3df931fe6979f2445c192cbfd59e04fd2d8a10f7c7573ac669f
4e549866ec1acadec4c84aaf8495992a28ec78d8ea5ef1b9f44dd843b0dcb7d4
O=C(c1ccccc1)N1CCCc2ccccc21
O=C(-O-C-c1:c:c:c:c:c:1)-[NH;D2;+0:1]-[C:2](-[C:3])-[c:4]>>[C:3]-[C:2](-[NH2;D1;+0:1])-[c:4]
92
[{"value": 92.0, "product": "CN(C1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N)C)C=C1)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 91.8, "product": "CN(C1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N)C)C=C1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
18
HOUR
(±)-Cis-[1-(4-dimethylamino-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-carbamic acid benzyl ester (665 mg, 1.49 mmol) was dissolved in ethanol (30 mL). The resulting solution was evacuated and backfilled with argon. A catalytic amount of palladium on carbon (10%) was added. The vessel was once again evacuated ...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether
Primary amine
c1ccccc1
null
c1ccc2c(c1)CCC[NH]2.c1ccccc1
HO-
C(C)O
null
18
C[C@H]1C[C@@H](NC(=O)OCc2ccccc2)c2ccccc2N1C(=O)c1ccc(N(C)C)cc1>C(C)O>C[C@H]1C[C@@H](N)c2ccccc2N1C(=O)c1ccc(N(C)C)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-96b71d3e08354fd7bf6e627018cf69a0
C[C@H]1C[C@@H](N)c2ccccc2N1C(=O)c1ccc(N(C)C)cc1.OB(O)c1ccc(Cl)cc1>>C[C@H]1C[C@@H](Nc2ccc(Cl)cc2)c2ccccc2N1C(=O)c1ccc(N(C)C)cc1
C(C)(=O)OCC.CN(C1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N)C)C=C1)C.ClC1=CC=C(C=C1)B(O)O.N1=CC=CC=C1>>CN(C1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)NC2=CC=C(C=C2)Cl)C)C=C1)C
[CH3:1][C@H:2]1[CH2:3][C@@H:4]([NH2:5])[c:13]2[cH:14][cH:15][cH:16][cH:17][c:18]2[N:19]1[C:20](=[O:21])[c:22]1[cH:23][cH:24][c:25]([N:26]([CH3:27])[CH3:28])[cH:29][cH:30]1.OB(O)[c:6]1[cH:7][cH:8][c:9]([Cl:10])[cH:11][cH:12]1>>[CH3:1][C@H:2]1[CH2:3][C@@H:4]([NH:5][c:6]2[cH:7][cH:8][c:9]([Cl:10])[cH:11][cH:12]2)[c:13]2[c...
C[C@H]1C[C@@H](N)c2ccccc2N1C(=O)c1ccc(N(C)C)cc1.OB(O)c1ccc(Cl)cc1
C[C@H]1C[C@@H](Nc2ccc(Cl)cc2)c2ccccc2N1C(=O)c1ccc(N(C)C)cc1
null
C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-]
CN(C)C=O
Heteroatom Alkylation and Arylation
Petasis reaction with amines and boronic acids
f5ae67a51de553a156f239a36ff1b30b0ec21b32d6467ebb95abe227e16748df
e74ce03b343a41c63fb42720bde3cd7e68ada25a9dc3f3bcf817625520d2a637
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
O-B(-O)-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[C:6]-[C:7](-[NH2;D1;+0:8])-[c:9]>>[C:6]-[C:7](-[NH;D2;+0:8]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5])-[c:9]
22
[{"value": 22.0, "product": "CN(C1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)NC2=CC=C(C=C2)Cl)C)C=C1)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 21.0, "product": "CN(C1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)NC2=CC=C(C=C2)Cl)C)C=C1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
1
HOUR
To a solution of (±)-cis-1-(4-dimethylamino-benzoyl)-2-methyl-1,2,3,4-tetrahydro-4-aminoquinoline (423 mg, 1.36 mmol) in DMF (15 mL, dry) was added 4-chlorophenylboronic acid (425 mg, 2.72 mmol), pyridine (322 mg, 330 uL, 4.08 mmol) and copper(II)acetate (494 mg, 2.72 mmol). The heterogeneous green mixture was stirred ...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Boronic acid
Secondary amine
c1ccccc1
c1ccccc1
c1ccccc1.c1ccc2c(c1)CCC[NH]2.c1ccccc1
HO-.B
C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-].CN(C)C=O
60
1
C[C@H]1C[C@@H](N)c2ccccc2N1C(=O)c1ccc(N(C)C)cc1.OB(O)c1ccc(Cl)cc1>C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-].CN(C)C=O>C[C@H]1C[C@@H](Nc2ccc(Cl)cc2)c2ccccc2N1C(=O)c1ccc(N(C)C)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-120369491031444abd6f94e7364ffc57
CC(=O)Cl.C[C@H]1C[C@@H](Nc2ccc(Cl)cc2)c2ccccc2N1C(=O)c1ccc(N(C)C)cc1>>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N(C)C)cc2)c2ccccc21
C(C)(=O)Cl.CN(C1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)NC2=CC=C(C=C2)Cl)C)C=C1)C.C(C)(C)N(CC)C(C)C>>ClC1=CC=C(C=C1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)N(C)C)=O)C
Cl[C:2]([CH3:1])=[O:3].[NH:4]([c:5]1[cH:6][cH:7][c:8]([Cl:9])[cH:10][cH:11]1)[C@@H:12]1[CH2:13][C@H:14]([CH3:15])[N:16]([C:17](=[O:18])[c:19]2[cH:20][cH:21][c:22]([N:23]([CH3:24])[CH3:25])[cH:26][cH:27]2)[c:28]2[cH:29][cH:30][cH:31][cH:32][c:33]21>>[CH3:1][C:2](=[O:3])[N:4]([c:5]1[cH:6][cH:7][c:8]([Cl:9])[cH:10][cH:11]...
CC(=O)Cl.C[C@H]1C[C@@H](Nc2ccc(Cl)cc2)c2ccccc2N1C(=O)c1ccc(N(C)C)cc1
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N(C)C)cc2)c2ccccc21
null
null
C(Cl)Cl
Acylation
N-alkylation of secondary amines with alkyl halides
b92e0bfd3d683c1f2a209adfe70a67ad7cb0d87749eb59e8fe0cf1689bc291e0
96cb0a2fed10552c5770a45a2d6523b47ac3e38928b4a9c698d8577451182dcd
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
Cl-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[C:4]-[C:5](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9])-[c:10]>>[C:4]-[C:5](-[N;H0;D3;+0:6](-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3])-[c:7](:[c:8]):[c:9])-[c:10]
34
[{"value": 34.0, "product": "ClC1=CC=C(C=C1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)N(C)C)=O)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
To a solution of (±)-cis-1-(4-dimethylamino-benzoyl)-2-methyl-1,2,3,4-tetrahydro-4-(N-4-chlorophenyl)aminoquinoline (120 mg, 0.29 mmol) in methylene chloride (2 mL) was added diisopropylethylamine (37 mg, 0.051 mL, 0.29 mmol) followed by acetyl chloride (2 mL). The mixture was stirred at rt 4 h. The mixture was concent...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Secondary amine
Tertiary amide
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HCl
C(Cl)Cl
null
4
CC(=O)Cl.C[C@H]1C[C@@H](Nc2ccc(Cl)cc2)c2ccccc2N1C(=O)c1ccc(N(C)C)cc1>C(Cl)Cl>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N(C)C)cc2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-fb8da0d1463e4b68b7ddae520b71cfb7
COc1cccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)c1>>COc1cccc(C(=O)N2c3ccccc3C(N(C(C)=O)c3ccc(Cl)cc3)CC2C)c1
ClC1=CC=C(C=C1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC(=CC=C1)OC)=O)C.CN(C1=CC=C(C(=O)Cl)C=C1)C>>ClC1=CC=C(C=C1)N(C(C)=O)C1CC(N(C2=CC=CC=C12)C(C1=CC(=CC=C1)OC)=O)C
[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7]([C:8](=[O:9])[N:10]2[c:11]3[cH:12][cH:13][cH:14][cH:15][c:16]3[C@H:17]([N:18]([C:19]([CH3:20])=[O:21])[c:22]3[cH:23][cH:24][c:25]([Cl:26])[cH:27][cH:28]3)[CH2:29][C@@H:30]2[CH3:31])[cH:32]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7]([C:8](=[O:9])[N:10]2[c:11]3[cH:12][cH:13][cH:...
COc1cccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)c1
COc1cccc(C(=O)N2c3ccccc3C(N(C(C)=O)c3ccc(Cl)cc3)CC2C)c1
null
null
null
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
O=C(c1ccccc1)N1CCC(Nc2ccccc2)c2ccccc21
null
null
[]
null
null
null
null
(±)-Cis-N-(4-chloro-phenyl)-N-[1-(3-methoxy-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-acetamide was made following general procedure B, substituting 3-methoxybenzoyl chloride for 4-dimethylaminobenzoyl chloride. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
null
null
null
null
COc1cccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)c1>>COc1cccc(C(=O)N2c3ccccc3C(N(C(C)=O)c3ccc(Cl)cc3)CC2C)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3480cf13a267421ab349ad761778e341
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(O)cc2)c2ccccc21.CCOC(=O)CCCBr>>CCOC(=O)CCCOc1ccc(C(=O)N2c3ccccc3[C@H](N(C(=O)CC)c3ccc(Cl)cc3)C[C@@H]2C)cc1
[H-].[Na+].C(C)O.ClC1=CC=C(C=C1)N(C(CC)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)O)=O)C.ClC1=CC=C(C=C1)N(C(CC)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)O)=O)C.BrCCCC(=O)OCC>>C(C)OC(CCCOC1=CC=C(C=C1)C(=O)N1[C@H](C[C@H](C2=CC=CC=C12)N(C(CC)=O)C1=CC=C(C=C1)Cl)C)=O
[OH:9][c:10]1[cH:11][cH:12][c:13]([C:14](=[O:15])[N:16]2[c:17]3[cH:18][cH:19][cH:20][cH:21][c:22]3[C@H:23]([N:24]([C:25](=[O:26])[CH2:27][CH3:28])[c:29]3[cH:30][cH:31][c:32]([Cl:33])[cH:34][cH:35]3)[CH2:36][C@@H:37]2[CH3:38])[cH:39][cH:40]1.Br[CH2:8][CH2:7][CH2:6][C:4]([O:3][CH2:2][CH3:1])=[O:5]>>[CH3:1][CH2:2][O:3][C:...
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(O)cc2)c2ccccc21.CCOC(=O)CCCBr
CCOC(=O)CCCOc1ccc(C(=O)N2c3ccccc3[C@H](N(C(=O)CC)c3ccc(Cl)cc3)C[C@@H]2C)cc1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
7e1040116e3a4cf0e8ec5cc7865388d9cd0efabce6d320a1c25a36e411018d8b
d5f4610d46ccc0478471c5bc0fb862644eaf764bbc5d93badb39d54f6ec8e0a5
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
Br-[CH2;D2;+0:1]-[C:2]-[C:3]-[C:4](-[#8:5])=[O;D1;H0:6].[OH;D1;+0:7]-[c:8](:[c:9]):[c:10]>>[#8:5]-[C:4](=[O;D1;H0:6])-[C:3]-[C:2]-[CH2;D2;+0:1]-[O;H0;D2;+0:7]-[c:8](:[c:9]):[c:10]
98
[{"value": 98.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
(±)-Cis-4-(4-{4-[(4-chloro-phenyl)-propionyl-amino]-2-methyl-3,4-dihydro-2H-quinoline-1-carbonyl}-phenoxy)-butyric acid ethyl ester was prepared from (±)-cis-N-(4-chloro-phenyl)-N-[1-(4-hydroxy-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-propionamide. (±)-Cis-N-(4-chloro-phenyl)-N-[1-(4-hydroxy-benzoyl)-2-methy...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic alcohol
Ether
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HBr
CN(C)C=O
null
0.5
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(O)cc2)c2ccccc21.CCOC(=O)CCCBr>CN(C)C=O>CCOC(=O)CCCOc1ccc(C(=O)N2c3ccccc3[C@H](N(C(=O)CC)c3ccc(Cl)cc3)C[C@@H]2C)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-71b3d92592b640719bd69b02e377bc0e
CCOC(=O)CCCOc1ccc(C(=O)N2c3ccccc3[C@H](N(C(=O)CC)c3ccc(Cl)cc3)C[C@@H]2C)cc1>>CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(OCCCC(=O)O)cc2)c2ccccc21
C(C)OC(CCCOC1=CC=C(C=C1)C(=O)N1[C@H](C[C@H](C2=CC=CC=C12)N(C(CC)=O)C1=CC=C(C=C1)Cl)C)=O.C(C)OC(CCCOC1=CC=C(C=C1)C(=O)N1[C@H](C[C@H](C2=CC=CC=C12)N(C(CC)=O)C1=CC=C(C=C1)Cl)C)=O.C([O-])([O-])=O.[K+].[K+]>>ClC1=CC=C(C=C1)N([C@@H]1C[C@@H](N(C2=CC=CC=C12)C(=O)C1=CC=C(OCCCC(=O)O)C=C1)C)C(CC)=O
CC[O:30][C:28]([CH2:27][CH2:26][CH2:25][O:24][c:23]1[cH:22][cH:21][c:20]([C:18]([N:17]2[C@@H:15]([CH3:16])[CH2:14][C@@H:13]([N:5]([C:3]([CH2:2][CH3:1])=[O:4])[c:6]3[cH:7][cH:8][c:9]([Cl:10])[cH:11][cH:12]3)[c:38]3[c:33]2[cH:34][cH:35][cH:36][cH:37]3)=[O:19])[cH:32][cH:31]1)=[O:29]>>[CH3:1][CH2:2][C:3](=[O:4])[N:5]([c:6...
CCOC(=O)CCCOc1ccc(C(=O)N2c3ccccc3[C@H](N(C(=O)CC)c3ccc(Cl)cc3)C[C@@H]2C)cc1
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(OCCCC(=O)O)cc2)c2ccccc21
null
null
O.CO
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
C-C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
31
[{"value": 31.0, "product": "ClC1=CC=C(C=C1)N([C@@H]1C[C@@H](N(C2=CC=CC=C12)C(=O)C1=CC=C(OCCCC(=O)O)C=C1)C)C(CC)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
(±)-Cis-4-(4-{4-[(4-chloro-phenyl)-propionyl-amino]-2-methyl-3,4-dihydro-2H-quinoline1-carbonyl}-phenoxy)-butyric acid was prepared from (±)-cis-4-(4-{4-[(4-chloro-phenyl)-propionyl-amino]-2-methyl-3,4-dihydro-2H-quinoline-1-carbonyl}-phenoxy)-butyric acid ethyl ester. Potassium carbonate (300 mg) was dissolved in wate...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
Other
O.CO
null
null
CCOC(=O)CCCOc1ccc(C(=O)N2c3ccccc3[C@H](N(C(=O)CC)c3ccc(Cl)cc3)C[C@@H]2C)cc1>O.CO>CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(OCCCC(=O)O)cc2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-51e47f6a1a494e2faa6806a79f4a4d80
CC(C)(CO)CBr.CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(O)cc2)c2ccccc21>>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(OCC(C)(C)CO)cc2)c2ccccc21
C([O-])([O-])=O.[K+].[K+].ClC1=CC=C(C=C1)N(C(CC)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)O)=O)C.ClC1=CC=C(C=C1)N(C(CC)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)O)=O)C.BrCC(CO)(C)C>>ClC1=CC=C(C=C1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OCC(CO)(C)C)=O)C
Br[CH2:24][C:25]([CH3:26])([CH3:27])[CH2:28][OH:29].C[CH2:1][C:2](=[O:3])[N:4]([c:5]1[cH:6][cH:7][c:8]([Cl:9])[cH:10][cH:11]1)[C@@H:12]1[CH2:13][C@H:14]([CH3:15])[N:16]([C:17](=[O:18])[c:19]2[cH:20][cH:21][c:22]([OH:23])[cH:30][cH:31]2)[c:32]2[cH:33][cH:34][cH:35][cH:36][c:37]21>>[CH3:1][C:2](=[O:3])[N:4]([c:5]1[cH:6][...
CC(C)(CO)CBr.CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(O)cc2)c2ccccc21
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(OCC(C)(C)CO)cc2)c2ccccc21
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
OtherReaction
7e1040116e3a4cf0e8ec5cc7865388d9cd0efabce6d320a1c25a36e411018d8b
d5f4610d46ccc0478471c5bc0fb862644eaf764bbc5d93badb39d54f6ec8e0a5
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
Br-[CH2;D2;+0:1]-[C:2](-[C:3])(-[C;D1;H3:4])-[C;D1;H3:5].C-[CH2;D2;+0:6]-[C:7](=[O;D1;H0:8])-[#7:9](-[C:10])-[c:11].[OH;D1;+0:12]-[c:13](:[c:14]):[c:15]>>[C:10]-[#7:9](-[c:11])-[C:7](-[CH3;D1;+0:6])=[O;D1;H0:8].[C:3]-[C:2](-[C;D1;H3:4])(-[C;D1;H3:5])-[CH2;D2;+0:1]-[O;H0;D2;+0:12]-[c:13](:[c:14]):[c:15]
44
[{"value": 44.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
95
CELSIUS
null
null
(±)-Cis-N-(4-chloro-phenyl)-N-{1-[4-(3-hydroxy-2,2-dimethyl-propoxy)-benzoyl]-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl}-acetamide was prepared from (±)-cis-N-(4-chloro-phenyl)-N-[1-(4-hydroxy-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-propionamide. (±)-Cis-N-(4-chloro-phenyl)-N-[1-(4-hydroxy-benzoyl)-2-methyl...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic alcohol
Ether
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HBr
CN(C)C=O
95
null
CC(C)(CO)CBr.CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(O)cc2)c2ccccc21>CN(C)C=O>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(OCC(C)(C)CO)cc2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f033a46294a4424e8a38ee9aaa52c684
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(O)cc2)c2ccccc21.COC(=O)C(C)(C)CBr>>COC(=O)C(C)(C)COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)cc1
COC(C(CBr)(C)C)=O.ClC1=CC=C(C=C1)N(C(CC)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)O)=O)C.ClC1=CC=C(C=C1)N(C(CC)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)O)=O)C.C([O-])([O-])=O.[K+].[K+]>>COC(C(COC1=CC=C(C=C1)C(=O)N1[C@H](C[C@H](C2=CC=CC=C12)N(C1=CC=C(C=C1)Cl)C(C)=O)C)(C)C)=O
C[CH2:26][C:25]([N:24]([C@H:23]1[c:22]2[c:17]([cH:18][cH:19][cH:20][cH:21]2)[N:16]([C:14]([c:13]2[cH:12][cH:11][c:10]([OH:9])[cH:39][cH:38]2)=[O:15])[C@@H:36]([CH3:37])[CH2:35]1)[c:28]1[cH:29][cH:30][c:31]([Cl:32])[cH:33][cH:34]1)=[O:27].Br[CH2:8][C:5]([C:3]([O:2][CH3:1])=[O:4])([CH3:6])[CH3:7]>>[CH3:1][O:2][C:3](=[O:4...
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(O)cc2)c2ccccc21.COC(=O)C(C)(C)CBr
COC(=O)C(C)(C)COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)cc1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
OtherReaction
7e1040116e3a4cf0e8ec5cc7865388d9cd0efabce6d320a1c25a36e411018d8b
d5f4610d46ccc0478471c5bc0fb862644eaf764bbc5d93badb39d54f6ec8e0a5
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
Br-[CH2;D2;+0:1]-[C:2](-[C;D1;H3:3])(-[C;D1;H3:4])-[C:5](=[O;D1;H0:6])-[#8:7]-[C;D1;H3:8].C-[CH2;D2;+0:9]-[C:10](=[O;D1;H0:11])-[#7:12](-[C:13])-[c:14].[OH;D1;+0:15]-[c:16](:[c:17]):[c:18]>>[C;D1;H3:8]-[#8:7]-[C:5](=[O;D1;H0:6])-[C:2](-[C;D1;H3:3])(-[C;D1;H3:4])-[CH2;D2;+0:1]-[O;H0;D2;+0:15]-[c:16](:[c:17]):[c:18].[C:1...
8
[{"value": 8.0, "product": "COC(C(COC1=CC=C(C=C1)C(=O)N1[C@H](C[C@H](C2=CC=CC=C12)N(C1=CC=C(C=C1)Cl)C(C)=O)C)(C)C)=O", "details": "PERCENTYIELD", "is_desired": false}]
95
CELSIUS
null
null
(±)-Cis-3-(4-{4-[acetyl-(4-chloro-phenyl)-amino]-2-methyl-3,4-dihydro-2H-quinoline-1-carbonyl}-phenoxy)-2,2-dimethyl-propionic acid methyl ester was prepared from (±)-cis-N-(4-chloro-phenyl)-N-[1-(4-hydroxy-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-propionamide. (±)-Cis-N-(4-chloro-phenyl)-N-[1-(4-hydroxy-ben...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic alcohol
Ether
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HBr
CN(C)C=O
95
null
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(O)cc2)c2ccccc21.COC(=O)C(C)(C)CBr>CN(C)C=O>COC(=O)C(C)(C)COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-32e3e8d4fa7245f6885e553fcbc5041c
CC(=O)Cl.COc1cccc(C(=O)N2c3ccccc3[C@H](Nc3ccccn3)C[C@@H]2C)c1>>COc1cccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccccn3)C[C@@H]2C)c1
COC=1C=C(C=CC1)C(=O)N1[C@H](C[C@H](C2=CC=CC=C12)NC1=NC=CC=C1)C.C(C)(=O)Cl>>COC=1C=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N(C(C)=O)C2=NC=CC=C2)C)C=CC1
Cl[C:19]([CH3:20])=[O:21].[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7]([C:8](=[O:9])[N:10]2[c:11]3[cH:12][cH:13][cH:14][cH:15][c:16]3[C@H:17]([NH:18][c:22]3[cH:23][cH:24][cH:25][cH:26][n:27]3)[CH2:28][C@@H:29]2[CH3:30])[cH:31]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7]([C:8](=[O:9])[N:10]2[c:11]3[cH:12][cH:13][cH:14][cH:...
CC(=O)Cl.COc1cccc(C(=O)N2c3ccccc3[C@H](Nc3ccccn3)C[C@@H]2C)c1
COc1cccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccccn3)C[C@@H]2C)c1
null
null
null
Acylation
N-alkylation of secondary amines with alkyl halides
b92e0bfd3d683c1f2a209adfe70a67ad7cb0d87749eb59e8fe0cf1689bc291e0
96cb0a2fed10552c5770a45a2d6523b47ac3e38928b4a9c698d8577451182dcd
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccn2)c2ccccc21
Cl-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[C:4]-[C:5](-[NH;D2;+0:6]-[c:7](:[c:8]):[#7;a:9]:[c:10])-[c:11]>>[C:4]-[C:5](-[N;H0;D3;+0:6](-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3])-[c:7](:[c:8]):[#7;a:9]:[c:10])-[c:11]
null
[]
null
null
null
null
Pd2(dba)3 (0.05 equ.), and rac-BINAP (0.1 equ.) were added to a flask with degassed toluene and stirred for 1 h. To the above solution was added 2-bromopyridine (1.1 equ.) and NaOtBu (1.1 equ.) and stirred for 30 min. (±)-Cis-(4-amino-2-methyl-3,4-dihydro-2H-quinolin-1-yl)-(3-methoxy-phenyl)-methanone was dissolved in ...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Secondary amine
Tertiary amide
null
null
c1ccccc1.c1ccncc1.c1ccc2c(c1)CCC[NH]2
HCl
null
null
null
CC(=O)Cl.COc1cccc(C(=O)N2c3ccccc3[C@H](Nc3ccccn3)C[C@@H]2C)c1>>COc1cccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccccn3)C[C@@H]2C)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-263b4f7f4c5245ea8effe447b074428c
CCC(=O)Cl.COc1cccc(C(=O)N2c3ccccc3[C@H](Nc3ccc(Cl)cn3)C[C@@H]2C)c1>>COc1cccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(Cl)cn3)C[C@@H]2C)c1
ClC=1C=CC(=NC1)N[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(=O)C1=CC(=CC=C1)OC)C.C(CC)(=O)Cl>>ClC=1C=CC(=NC1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC(=CC=C1)OC)=O)C
C[CH2:20][C:19](Cl)=[O:21].[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7]([C:8](=[O:9])[N:10]2[c:11]3[cH:12][cH:13][cH:14][cH:15][c:16]3[C@H:17]([NH:18][c:22]3[cH:23][cH:24][c:25]([Cl:26])[cH:27][n:28]3)[CH2:29][C@@H:30]2[CH3:31])[cH:32]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7]([C:8](=[O:9])[N:10]2[c:11]3[cH:12][cH:13][c...
CCC(=O)Cl.COc1cccc(C(=O)N2c3ccccc3[C@H](Nc3ccc(Cl)cn3)C[C@@H]2C)c1
COc1cccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(Cl)cn3)C[C@@H]2C)c1
null
null
null
Acylation
OtherReaction
b92e0bfd3d683c1f2a209adfe70a67ad7cb0d87749eb59e8fe0cf1689bc291e0
96cb0a2fed10552c5770a45a2d6523b47ac3e38928b4a9c698d8577451182dcd
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccn2)c2ccccc21
C-[CH2;D2;+0:1]-[C;H0;D3;+0:2](-Cl)=[O;D1;H0:3].[C:4]-[C:5](-[NH;D2;+0:6]-[c:7](:[c:8]):[#7;a:9]:[c:10])-[c:11]>>[C:4]-[C:5](-[N;H0;D3;+0:6](-[C;H0;D3;+0:2](-[CH3;D1;+0:1])=[O;D1;H0:3])-[c:7](:[c:8]):[#7;a:9]:[c:10])-[c:11]
null
[]
null
null
null
null
To a flask was added Pd2(dba)3 (molar 0.05 equ.), and rac-BINAP (0.1 equ.) in degassed toluene and stirred for 1 h. To the above solution was added 2,5-dichloropyridinepyridine (1.1 equ.) and NaOtBu (1.1 equ.) and stirred for 30 min. The corresponding amine, (±)-cis-(4-amino-2-methyl-3,4-dihydro-2H-quinolin-1-yl)-(3-me...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Secondary amine
Tertiary amide
null
null
c1ccccc1.c1ccncc1.c1ccc2c(c1)CCC[NH]2
HCl
null
null
null
CCC(=O)Cl.COc1cccc(C(=O)N2c3ccccc3[C@H](Nc3ccc(Cl)cn3)C[C@@H]2C)c1>>COc1cccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(Cl)cn3)C[C@@H]2C)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-38ef0511f95740f39c826894bf1ee9e4
COc1ccc(C(=O)N2c3cccc(C)c3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)cc1>>COc1ccc(C(=O)N2c3cc(C)ccc3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)cc1
CN(C1=CC=C(C(=O)Cl)C=C1)C.ClC1=CC=C(C=C1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC(=C12)C)C(C1=CC=C(C=C1)OC)=O)C.NC1=CC=CC=C1.COC1=CC=C(C(=O)Cl)C=C1>>ClC1=CC=C(C=C1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC(=CC=C12)C)C(C1=CC=C(C=C1)OC)=O)C
[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([C:7](=[O:8])[N:9]2[c:10]3[cH:11][cH:15][cH:14][c:12]([CH3:13])[c:16]3[C@H:17]([N:18]([C:19]([CH3:20])=[O:21])[c:22]3[cH:23][cH:24][c:25]([Cl:26])[cH:27][cH:28]3)[CH2:29][C@@H:30]2[CH3:31])[cH:32][cH:33]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([C:7](=[O:8])[N:9]2[c:10]3[cH:11][c:12]([C...
COc1ccc(C(=O)N2c3cccc(C)c3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)cc1
COc1ccc(C(=O)N2c3cc(C)ccc3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)cc1
null
null
null
Miscellaneous
OtherReaction
79503c5bbd93d082bf8197f3441c50e1f6cf2c3dcd153866fb3370eae24e26fc
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
[C;D1;H3:1]-[c;H0;D3;+0:2]1:[c:3]:[cH;D2;+0:4]:[cH;D2;+0:5]:[c:6]2:[c;H0;D3;+0:7]:1-[C:8](-[#7:9]-[C:10](-[C;D1;H3:11])=[O;D1;H0:12])-[C:13]-[C:14]-[#7:15]-2-[C:16]=[O;D1;H0:17]>>[C;D1;H3:1]-[c;H0;D3;+0:2]1:[c:3]:[cH;D2;+0:4]:[c;H0;D3;+0:7]2:[c:6](:[cH;D2;+0:5]:1)-[#7:15](-[C:16]=[O;D1;H0:17])-[C:14]-[C:13]-[C:8]-2-[#7...
null
[]
null
null
null
null
(±)-Cis-N-(4-chloro-phenyl)-N-[1-(4-methoxy-benzoyl)-2,5-dimethyl-1,2,3,4-tetrahydro-quinolin-4-yl]-acetamide was made following general procedure B, substituting 3-toluidine for aniline and 4-methoxybenzoyl chloride for 4-dimethylaminobenzoyl chloride. The reaction was non-selective and also (±)-cis-N-(4-chloro-phenyl...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ccc2c(c1)CCC[NH]2
c1ccc2c(c1)CCC[NH]2
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
null
null
null
null
COc1ccc(C(=O)N2c3cccc(C)c3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)cc1>>COc1ccc(C(=O)N2c3cc(C)ccc3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e910182a178145818307b5e304d64f29
CN(C)c1ccc(C(=O)Cl)cc1.COc1ccc(C(=O)Cl)cc1.Nc1ccccc1>>COc1ccc(C(=O)N2c3cccc(C)c3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)cc1
COC1=CC=C(C(=O)Cl)C=C1.ClC1=CC=C(C=C1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC(=CC=C12)C)C(C1=CC=C(C=C1)OC)=O)C.CN(C1=CC=C(C(=O)Cl)C=C1)C.NC1=CC=CC=C1>>ClC1=CC=C(C=C1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC(=C12)C)C(C1=CC=C(C=C1)OC)=O)C.ClC1=CC=C(C=C1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC(=CC=C12)C)C(C1=CC=C(C=C1)OC)=O)C
[C:48](=[O:54])([c:58]1[cH:57][cH:56][c:55]([N:51]([CH3:50])[CH3:53])[cH:61][cH:60]1)[Cl:59].Cl[C:40]([c:39]1[cH:38][cH:37][c:36]([O:35][CH3:34])[cH:66][cH:65]1)=[O:41].[NH2:42][c:43]1[cH:44][cH:45][cH:46][cH:47][cH:49]1>>[CH3:34][O:35][c:36]1[cH:37][cH:38][c:39]([C:40](=[O:41])[N:42]2[c:43]3[cH:44][cH:45][cH:46][c:47]...
CN(C)c1ccc(C(=O)Cl)cc1.COc1ccc(C(=O)Cl)cc1.Nc1ccccc1
COc1ccc(C(=O)N2c3cccc(C)c3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)cc1
null
null
null
Acylation
OtherReaction
c02605f28509cb45c0705e3739d0c93f15e46daff81767c35772be1a402979f0
727332e0bdbab460e01b92629aaea07cc604a97aa6e2606a2b027cd820543559
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[CH3;D1;+0:6]-[N;H0;D3;+0:7](-[CH3;D1;+0:8])-[c:9]1:[c:10]:[c:11]:[c;H0;D3;+0:12](-[C;H0;D3;+0:13](-[Cl;H0;D1;+0:14])=[O;H0;D1;+0:15]):[c:16]:[c:17]:1.[NH2;D1;+0:18]-[c:19]1:[c:20]:[c:21]:[c:22]:[cH;D2;+0:23]:[cH;D2;+0:24]:1>>[C;D1;H3:25]-[C:26]1-[C:27]-[C@@H;D3;+0:6]...
null
[]
null
null
null
null
(±)-Cis-N-(4-chloro-phenyl)-N-[1-(4-methoxy-benzoyl)-2,7-dimethyl-1,2,3,4-tetrahydro-quinolin-4-yl]-acetamide was made following general procedure B, substituting 3-toluidine for aniline and 4-methoxybenzoyl chloride for 4-dimethylaminobenzoyl chloride. The reaction was non-selective, and also (±)-cis-N-(4-chloro-pheny...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Acyl halide.Primary amine.Tertiary amine
Aromatic halide.Tertiary amide.Tertiary amide
c1ccccc1.c1ccccc1
c1ccccc1.c1ccc2c(c1)CCC[NH]2
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
null
null
null
null
CN(C)c1ccc(C(=O)Cl)cc1.COc1ccc(C(=O)Cl)cc1.Nc1ccccc1>>COc1ccc(C(=O)N2c3cccc(C)c3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1a23ecf6bd324c0486f05fa17bd820c7
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(OCC(=O)OC)cc21>>CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(OCC(=O)O)cc21
COC(COC=1C=C2[C@@H](C[C@@H](N(C2=CC1)C(C1=CC=C(C=C1)F)=O)C)N(C(CC)=O)C1=CC=C(C=C1)Cl)=O.COC(COC=1C=C2[C@@H](C[C@@H](N(C2=CC1)C(C1=CC=C(C=C1)F)=O)C)N(C(CC)=O)C1=CC=C(C=C1)Cl)=O.[OH-].[Na+]>>ClC1=CC=C(C=C1)N([C@@H]1C[C@@H](N(C2=CC=C(C=C12)OCC(=O)O)C(C1=CC=C(C=C1)F)=O)C)C(CC)=O
C[O:35][C:33]([CH2:32][O:31][c:30]1[cH:29][cH:28][c:27]2[c:37]([cH:36]1)[C@H:13]([N:5]([C:3]([CH2:2][CH3:1])=[O:4])[c:6]1[cH:7][cH:8][c:9]([Cl:10])[cH:11][cH:12]1)[CH2:14][C@H:15]([CH3:16])[N:17]2[C:18](=[O:19])[c:20]1[cH:21][cH:22][c:23]([F:24])[cH:25][cH:26]1)=[O:34]>>[CH3:1][CH2:2][C:3](=[O:4])[N:5]([c:6]1[cH:7][cH:...
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(OCC(=O)OC)cc21
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(OCC(=O)O)cc21
null
null
CO
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
94
[{"value": 94.0, "product": "ClC1=CC=C(C=C1)N([C@@H]1C[C@@H](N(C2=CC=C(C=C12)OCC(=O)O)C(C1=CC=C(C=C1)F)=O)C)C(CC)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
(±)-Cis-[4-[(4-chloro-phenyl)-propionyl-amino]-1-(4-fluoro-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-6-yloxy]-acetic acid was prepared from (±)-cis-[4-[(4-chloro-phenyl)-propionyl-amino]-1-(4-fluoro-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-6-yloxy]-acetic acid methyl ester. To a solution of (±)-cis-[4-[(4-chlo...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
Other
CO
null
3
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(OCC(=O)OC)cc21>CO>CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(OCC(=O)O)cc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-50b82e49bcce46dd8ab596a9d676d6fe
CCOC(=O)C(C)(C)Oc1ccc2c(c1)[C@H](N(C(=O)CC)c1ccc(Cl)cc1)C[C@H](C)N2C(=O)c1ccc(F)cc1>>CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(OC(C)(C)C(=O)O)cc21
ClC1=CC=C(C=C1)N([C@@H]1C[C@@H](N(C2=CC=C(C=C12)OCC(=O)O)C(C1=CC=C(C=C1)F)=O)C)C(CC)=O.C(C)OC(C(C)(C)OC=1C=C2[C@@H](C[C@@H](N(C2=CC1)C(C1=CC=C(C=C1)F)=O)C)N(C(CC)=O)C1=CC=C(C=C1)Cl)=O>>ClC1=CC=C(C=C1)N([C@@H]1C[C@@H](N(C2=CC=C(C=C12)OC(C(=O)O)(C)C)C(C1=CC=C(C=C1)F)=O)C)C(CC)=O
CC[O:37][C:35]([C:32]([O:31][c:30]1[cH:29][cH:28][c:27]2[c:39]([cH:38]1)[C@H:13]([N:5]([C:3]([CH2:2][CH3:1])=[O:4])[c:6]1[cH:7][cH:8][c:9]([Cl:10])[cH:11][cH:12]1)[CH2:14][C@H:15]([CH3:16])[N:17]2[C:18](=[O:19])[c:20]1[cH:21][cH:22][c:23]([F:24])[cH:25][cH:26]1)([CH3:33])[CH3:34])=[O:36]>>[CH3:1][CH2:2][C:3](=[O:4])[N:...
CCOC(=O)C(C)(C)Oc1ccc2c(c1)[C@H](N(C(=O)CC)c1ccc(Cl)cc1)C[C@H](C)N2C(=O)c1ccc(F)cc1
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(OC(C)(C)C(=O)O)cc21
null
null
null
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
C-C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
null
[]
null
null
null
null
(±)-Cis-2-[4-[(4-chloro-phenyl)-propionyl-amino]-1-(4-fluoro-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-6-yloxy]-2-methyl-propionic acid was prepared from (±)-cis-2-[4-[(4-chloro-phenyl)-propionyl-amino]-1-(4-fluoro-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-6-yloxy]-2-methyl-propionic acid ethyl ester. The sapon...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
Other
null
null
null
CCOC(=O)C(C)(C)Oc1ccc2c(c1)[C@H](N(C(=O)CC)c1ccc(Cl)cc1)C[C@H](C)N2C(=O)c1ccc(F)cc1>>CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(OC(C)(C)C(=O)O)cc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c7dd50cda3cc4df084e203a5b26f899c
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(OCC(=O)OC)cc21.N>>CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(OCC(N)=O)cc21
COC(COC=1C=C2[C@@H](C[C@@H](N(C2=CC1)C(C1=CC=C(C=C1)F)=O)C)N(C(CC)=O)C1=CC=C(C=C1)Cl)=O.N>>C(N)(=O)COC=1C=C2[C@@H](C[C@@H](N(C2=CC1)C(C1=CC=C(C=C1)F)=O)C)N(C(CC)=O)C1=CC=C(C=C1)Cl
CO[C:33]([CH2:32][O:31][c:30]1[cH:29][cH:28][c:27]2[c:37]([cH:36]1)[C@H:13]([N:5]([C:3]([CH2:2][CH3:1])=[O:4])[c:6]1[cH:7][cH:8][c:9]([Cl:10])[cH:11][cH:12]1)[CH2:14][C@H:15]([CH3:16])[N:17]2[C:18](=[O:19])[c:20]1[cH:21][cH:22][c:23]([F:24])[cH:25][cH:26]1)=[O:35].[NH3:34]>>[CH3:1][CH2:2][C:3](=[O:4])[N:5]([c:6]1[cH:7]...
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(OCC(=O)OC)cc21.N
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(OCC(N)=O)cc21
null
null
CO
Acylation
OtherReaction
d5b10d4f469e7a196a3b04a6a9e159a7d90514b6df5b50c1197d4b1b774c04e1
adc0ef6f6c1340dd2dbab737c85bf17fc842769181c5db1a2b4f82b391b28f9f
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#8:4].[NH3;D0;+0:5]>>[#8:4]-[C:3]-[C;H0;D3;+0:1](-[NH2;D1;+0:5])=[O;D1;H0:2]
76
[{"value": 76.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
(±)-Cis-N-[6-carbamoylmethoxy-1-(4-fluoro-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-N-(4-chloro-phenyl)-propionamide was prepared from (±)-cis-4-[(4-chloro-phenyl)-propionyl-amino]-1-(4-fluoro-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-6-yloxy]-acetic acid ester. To solid (±)-cis-[4-[(4-chloro-phenyl)-prop...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary amide
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HO-
CO
null
null
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(OCC(=O)OC)cc21.N>CO>CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(OCC(N)=O)cc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9db6d5d4165a41d9a889c82f20e21d81
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(N3CCOCC3)cc21.CCC(=O)N(c1ccc(N(CC)CC)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(N(CC)CC)cc21>>CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(N(CC)CC)cc21
N1CCOCC1.C(C)N(C=1C=C2[C@@H](C[C@@H](N(C2=CC1)C(C1=CC=C(C=C1)F)=O)C)N(C(CC)=O)C1=CC=C(C=C1)N(CC)CC)CC.ClC1=CC=C(C=C1)N(C(CC)=O)[C@@H]1C[C@@H](N(C2=CC=C(C=C12)N1CCOCC1)C(C1=CC=C(C=C1)F)=O)C.C(C)NCC>>ClC1=CC=C(C=C1)N(C(CC)=O)[C@@H]1C[C@@H](N(C2=CC=C(C=C12)N(CC)CC)C(C1=CC=C(C=C1)F)=O)C
C1C[N:31]([c:30]2[cH:29][cH:28][c:27]3[c:37]([cH:36]2)[C@H:13]([N:5]([C:3]([CH2:2][CH3:1])=[O:4])[c:6]2[cH:7][cH:8][c:9]([Cl:10])[cH:11][cH:12]2)[CH2:14][C@H:15]([CH3:16])[N:17]3[C:18](=[O:19])[c:20]2[cH:21][cH:22][c:23]([F:24])[cH:25][cH:26]2)CCO1.CCC(=O)N(c1ccc(N(CC)CC)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(N([...
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(N3CCOCC3)cc21.CCC(=O)N(c1ccc(N(CC)CC)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(N(CC)CC)cc21
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(N(CC)CC)cc21
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
efd76e2963b786dd6171a8a72562617283a1971e96ecbb3998266ebedcfc7125
c53cfac120282988daea7947474e4981c55c68780205307a9609d5cf214b3a48
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
C-C-C(=O)-N(-[C@H]1-C-[C@H](-C)-N(-C(=O)-c2:c:c:c(-F):c:c:2)-c2:c:c:c(-N(-[CH2;D2;+0:1]-[C;D1;H3:2])-[CH2;D2;+0:3]-[C;D1;H3:4]):c:c:2-1)-c1:c:c:c(-N(-C-C)-C-C):c:c:1.[c:5]:[c:6](-[N;H0;D3;+0:7]1-C-C-O-C-C-1):[c:8]>>[C;D1;H3:2]-[CH2;D2;+0:1]-[N;H0;D3;+0:7](-[CH2;D2;+0:3]-[C;D1;H3:4])-[c:6](:[c:5]):[c:8]
null
[]
null
null
null
null
(±)-Cis-N-[6-diethylamino-1-(4-fluoro-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-N(4-diethylamino-phenyl)-propionamide was made in the same way as (±)-cis-N-(4-chloro-phenyl)-N-[1 -(4-fluoro-benzoyl)-2-methyl-6-morpholin-4-yl-1,2,3,4-tetrahydro-quinolin-4-yl]-propionamide except diethylamine was substituted fo...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ether.Tertiary amide.Tertiary amide.Tertiary amine.Tertiary amine.Tertiary amine
Tertiary amine
C1COCC[NH]1.c1ccccc1.c1ccccc1.c1ccc2c(c1)CCCN2
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HF
null
null
null
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(N3CCOCC3)cc21.CCC(=O)N(c1ccc(N(CC)CC)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(N(CC)CC)cc21>>CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(N(CC)CC)cc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7f80f4ca960246edae8c256394ee132e
C=CC(=O)OC.CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(C=CC(=O)O)cc21>>CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(C=CC(=O)OC)cc21
ClC1=CC=C(C=C1)N([C@@H]1C[C@@H](N(C2=CC=C(C=C12)C=CC(=O)O)C(C1=CC=C(C=C1)F)=O)C)C(CC)=O.BrC=1C=C2[C@@H](C[C@@H](N(C2=CC1)C(C1=CC=C(C=C1)F)=O)C)N(C(CC)=O)C1=CC=C(C=C1)Cl.BrC=1C=C2[C@@H](C[C@@H](N(C2=CC1)C(C1=CC=C(C=C1)F)=O)C)N(C(CC)=O)C1=CC=C(C=C1)Cl.C1(=CC=CC=C1)P(CCCP(C1=CC=CC=C1)C1=CC=CC=C1)C1=CC=CC=C1.C(C=C)(=O)OC>>...
[CH2:31]=[CH:32][C:33](=[O:34])[O:35][CH3:36].O=C(O)C=C[c:30]1[cH:29][cH:28][c:27]2[c:38]([cH:37]1)[C@H:13]([N:5]([C:3]([CH2:2][CH3:1])=[O:4])[c:6]1[cH:7][cH:8][c:9]([Cl:10])[cH:11][cH:12]1)[CH2:14][C@H:15]([CH3:16])[N:17]2[C:18](=[O:19])[c:20]1[cH:21][cH:22][c:23]([F:24])[cH:25][cH:26]1>>[CH3:1][CH2:2][C:3](=[O:4])[N:...
C=CC(=O)OC.CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(C=CC(=O)O)cc21
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(C=CC(=O)OC)cc21
null
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-]
CN(C)C=O
C-C Coupling
O-methylation
4e23d12bae162def895de92701734e7f85ca2550b29fa0799f377287203cdcfc
271e3ba7f993df4472e473adf24569183d3aab0b5124850797c108a882536876
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
O-C(=O)-C=C-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[C;D1;H3:6]-[#8:7]-[C:8](=[O;D1;H0:9])-[C:10]=[CH2;D1;+0:11]>>[C;D1;H3:6]-[#8:7]-[C:8](=[O;D1;H0:9])-[C:10]=[CH;D2;+0:11]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
44
[{"value": 44.0, "product": "COC(C=CC=1C=C2[C@@H](C[C@@H](N(C2=CC1)C(C1=CC=C(C=C1)F)=O)C)N(C(CC)=O)C1=CC=C(C=C1)Cl)=O", "details": "PERCENTYIELD", "is_desired": false}]
80
CELSIUS
null
null
(±)-Cis-3-[4-[(4-chloro-phenyl)-propionyl-amino]-1-(4-fluoro-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-6-yl]-acrylic acid was made from (±)-cis-N-[6-bromo-1-(4-fluoro-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-N-(4-chloro-phenyl)-propionamide. To a solution of (±)-cis-N-[6-bromo-1-(4-fluoro-benzoyl)-2-meth...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Vinyl
null
c1ccc2c(c1)CCC[NH]2
c1ccc2c(c1)CCC[NH]2
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HO-
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].CN(C)C=O
80
null
C=CC(=O)OC.CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(C=CC(=O)O)cc21>C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].CN(C)C=O>CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(C=CC(=O)OC)cc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f314d735920a44cca0e0786ce89d3265
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(C=CC(=O)OC)cc21>>CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(C=CC(=O)O)cc21
COC(C=CC=1C=C2[C@@H](C[C@@H](N(C2=CC1)C(C1=CC=C(C=C1)F)=O)C)N(C(CC)=O)C1=CC=C(C=C1)Cl)=O.C(=O)([O-])[O-].[K+].[K+]>>ClC1=CC=C(C=C1)N([C@@H]1C[C@@H](N(C2=CC=C(C=C12)C=CC(=O)O)C(C1=CC=C(C=C1)F)=O)C)C(CC)=O
C[O:35][C:33]([CH:32]=[CH:31][c:30]1[cH:29][cH:28][c:27]2[c:37]([cH:36]1)[C@H:13]([N:5]([C:3]([CH2:2][CH3:1])=[O:4])[c:6]1[cH:7][cH:8][c:9]([Cl:10])[cH:11][cH:12]1)[CH2:14][C@H:15]([CH3:16])[N:17]2[C:18](=[O:19])[c:20]1[cH:21][cH:22][c:23]([F:24])[cH:25][cH:26]1)=[O:34]>>[CH3:1][CH2:2][C:3](=[O:4])[N:5]([c:6]1[cH:7][cH...
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(C=CC(=O)OC)cc21
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(C=CC(=O)O)cc21
null
null
O.CO
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[C:4]=[C:5]-[c:6]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[C:4]=[C:5]-[c:6]
9.1
[{"value": 9.1, "product": "ClC1=CC=C(C=C1)N([C@@H]1C[C@@H](N(C2=CC=C(C=C12)C=CC(=O)O)C(C1=CC=C(C=C1)F)=O)C)C(CC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To a solution of (±)-cis-3-[4-[(4-chloro-phenyl)-propionyl-amino]-1-(4-fluoro-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-6-yl]-acrylic acid methyl ester (110 mg, 0.21 mmol) in 4 ml methanol was added 50 mg K2CO3, (0.36 mmol, in 2 ml water). The resulting reaction mixture was stirred at room temperature overnight. Th...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
Other
O.CO
null
8
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(C=CC(=O)OC)cc21>O.CO>CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(C=CC(=O)O)cc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-54ae29eb40e94ac4b695192d33829aa6
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N(C)C)cc2)c2cc(N3CCOCC3)ccc21.CCN(CC)c1ccc(N(C(C)=O)[C@@H]2C[C@H](C)N(C(=O)c3ccc(N(C)C)cc3)c3cc(N(CC)CC)ccc32)cc1.CCNCC>>CCN(CC)c1ccc2c(c1)N(C(=O)c1ccc(N(C)C)cc1)[C@@H](C)C[C@H]2N(C(C)=O)c1ccc(Cl)cc1
N1CCOCC1.C(C)N(C1=CC=C2[C@@H](C[C@@H](N(C2=C1)C(C1=CC=C(C=C1)N(C)C)=O)C)N(C(C)=O)C1=CC=C(C=C1)N(CC)CC)CC.ClC1=CC=C(C=C1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC(=CC=C12)N1CCOCC1)C(C1=CC=C(C=C1)N(C)C)=O)C.C(C)NCC>>ClC1=CC=C(C=C1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC(=CC=C12)N(CC)CC)C(C1=CC=C(C=C1)N(C)C)=O)C
C1C[N:3]([c:6]2[cH:7][cH:8][c:9]3[c:10]([cH:11]2)[N:12]([C:13](=[O:14])[c:15]2[cH:16][cH:17][c:18]([N:19]([CH3:20])[CH3:21])[cH:22][cH:23]2)[C@@H:24]([CH3:25])[CH2:26][C@H:27]3[N:28]([C:29]([CH3:30])=[O:31])[c:32]2[cH:33][cH:34][c:35]([Cl:36])[cH:37][cH:38]2)CCO1.CCN(CC)c1ccc(N(C(C)=O)[C@@H]2C[C@H](C)N(C(=O)c3ccc(N(C)C...
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N(C)C)cc2)c2cc(N3CCOCC3)ccc21.CCN(CC)c1ccc(N(C(C)=O)[C@@H]2C[C@H](C)N(C(=O)c3ccc(N(C)C)cc3)c3cc(N(CC)CC)ccc32)cc1.CCNCC
CCN(CC)c1ccc2c(c1)N(C(=O)c1ccc(N(C)C)cc1)[C@@H](C)C[C@H]2N(C(C)=O)c1ccc(Cl)cc1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
11d320f23afe6af73b55c140707bb309928e9754a7f161babb31980236480ee6
a231863537e19cc9af31abf5655fd391c5eedc0dcaffbdb0906d38ebe6000b4b
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
C-C-N(-C-C)-c1:c:c:c(-N(-C(-C)=O)-[C@H]2-C-[C@H](-C)-N(-C(=O)-c3:c:c:c(-N(-C)-C):c:c:3)-c3:c:c(-N(-C-C)-[CH2;D2;+0:1]-[C;D1;H3:2]):c:c:c:3-2):c:c:1.C-C-N-[CH2;D2;+0:3]-[C;D1;H3:4].[c:5]:[c:6](-[N;H0;D3;+0:7]1-C-C-O-C-C-1):[c:8]>>[C;D1;H3:4]-[CH2;D2;+0:3]-[N;H0;D3;+0:7](-[CH2;D2;+0:1]-[C;D1;H3:2])-[c:6](:[c:5]):[c:8]
null
[]
null
null
null
null
(±)-Cis-N-[7-diethylamino-1-(4-dimethylamino-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-N-(4-diethylamino-phenyl)-acetamide was made in the same way as (±)-cis-N-(4-chloro-phenyl)-N-[1-(4-dimethylamino-benzoyl)-2-methyl-7-morpholin-4-yl-1,2,3,4-tetrahydro-quinolin-4-yl]-acetamide except diethylamine was substi...
10.6084/m9.figshare.5104873.v1
null
Ether.Tertiary amide.Tertiary amide.Secondary amine.Tertiary amine.Tertiary amine.Tertiary amine.Tertiary amine
Tertiary amine
C1COCC[NH]1.c1ccccc1.c1ccccc1.c1ccc2c(c1)CCCN2
null
c1ccccc1.c1ccc2c(c1)CCC[NH]2.c1ccccc1
HO-
null
null
null
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N(C)C)cc2)c2cc(N3CCOCC3)ccc21.CCN(CC)c1ccc(N(C(C)=O)[C@@H]2C[C@H](C)N(C(=O)c3ccc(N(C)C)cc3)c3cc(N(CC)CC)ccc32)cc1.CCNCC>>CCN(CC)c1ccc2c(c1)N(C(=O)c1ccc(N(C)C)cc1)[C@@H](C)C[C@H]2N(C(C)=O)c1ccc(Cl)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f15c55a7229a43138f1c1bb39467f81b
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N(C)C)cc2)c2cc(O)ccc21.CCOC(=O)CCCBr>>CCOC(=O)COc1ccc2c(c1)N(C(=O)c1ccc(N(C)C)cc1)[C@@H](C)C[C@H]2N(C(C)=O)c1ccc(Cl)cc1
C(C)OC(CCCOC1=CC=C(C=C1)C(=O)N1[C@H](C[C@H](C2=CC=CC=C12)N(C(CC)=O)C1=CC=C(C=C1)Cl)C)=O.ClC1=CC=C(C=C1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC(=CC=C12)O)C(C1=CC=C(C=C1)N(C)C)=O)C.BrCCCC(=O)OCC>>C(C)OC(COC1=CC=C2[C@@H](C[C@@H](N(C2=C1)C(C1=CC=C(C=C1)N(C)C)=O)C)N(C1=CC=C(C=C1)Cl)C(C)=O)=O
[OH:7][c:8]1[cH:9][cH:10][c:11]2[c:12]([cH:13]1)[N:14]([C:15](=[O:16])[c:17]1[cH:18][cH:19][c:20]([N:21]([CH3:22])[CH3:23])[cH:24][cH:25]1)[C@@H:26]([CH3:27])[CH2:28][C@H:29]2[N:30]([C:31]([CH3:32])=[O:33])[c:34]1[cH:35][cH:36][c:37]([Cl:38])[cH:39][cH:40]1.BrCC[CH2:6][C:4]([O:3][CH2:2][CH3:1])=[O:5]>>[CH3:1][CH2:2][O:...
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N(C)C)cc2)c2cc(O)ccc21.CCOC(=O)CCCBr
CCOC(=O)COc1ccc2c(c1)N(C(=O)c1ccc(N(C)C)cc1)[C@@H](C)C[C@H]2N(C(C)=O)c1ccc(Cl)cc1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
50d675b335c583a6ce22e1164b27a78b18b9ca447d45137820c344bcb6369217
0865de4e1853c59ac25437e36fd18b03329566cb9eff4b4f0ce70d5714692fd3
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
Br-C-C-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#8:4]-[C:5].[OH;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[C:5]-[#8:4]-[C:2](=[O;D1;H0:3])-[CH2;D2;+0:1]-[O;H0;D2;+0:6]-[c:7](:[c:8]):[c:9]
null
[]
null
null
null
null
(±)-Cis-[4-[acetyl-(4-chloro-phenyl)-amino]-1-(4-dimethylamino-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-7-yloxy]-acetic acid ethyl ester was prepared from (±)-cis-N-(4-chloro-phenyl)-N-[1-(4-dimethylamino-benzoyl)-7-hydroxy-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-acetamide, following the alkylation conditions d...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester.Aromatic alcohol
Ester.Ether
null
null
c1ccccc1.c1ccc2c(c1)CCC[NH]2.c1ccccc1
HBr
null
null
null
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N(C)C)cc2)c2cc(O)ccc21.CCOC(=O)CCCBr>>CCOC(=O)COc1ccc2c(c1)N(C(=O)c1ccc(N(C)C)cc1)[C@@H](C)C[C@H]2N(C(C)=O)c1ccc(Cl)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-69c1f7f68d5c4a3da58579363c6ad4b0
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(OCC(N)=O)cc21.CCOC(=O)COc1ccc2c(c1)N(C(=O)c1ccc(N(C)C)cc1)[C@@H](C)C[C@H]2N(C(C)=O)c1ccc(Cl)cc1>>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N(C)C)cc2)c2cc(OCC(N)=O)ccc21
C(N)(=O)COC=1C=C2[C@@H](C[C@@H](N(C2=CC1)C(C1=CC=C(C=C1)F)=O)C)N(C(CC)=O)C1=CC=C(C=C1)Cl.C(C)OC(COC1=CC=C2[C@@H](C[C@@H](N(C2=C1)C(C1=CC=C(C=C1)N(C)C)=O)C)N(C1=CC=C(C=C1)Cl)C(C)=O)=O>>C(C)(=O)N([C@@H]1C[C@@H](N(C2=CC(=CC=C12)OCC(=O)N)C(C1=CC=C(C=C1)N(C)C)=O)C)C1=CC=C(C=C1)Cl
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)[c:38]2[c:28]1[cH:29][c:30]([O:31][CH2:32][C:33]([NH2:34])=[O:35])[cH:36][cH:37]2.CCOC(=O)COc1ccc2c(c1)[N:16]([C:17](=[O:18])[c:19]1[cH:20][cH:21][c:22]([N:23]([CH3:24])[CH3:25])[cH:26][cH:27]1)[C@@H:14]([CH3:15])[CH2:13][C@H:12]2[N:4]([C:2]([CH3:1])=[O:3])[c:5]1...
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(OCC(N)=O)cc21.CCOC(=O)COc1ccc2c(c1)N(C(=O)c1ccc(N(C)C)cc1)[C@@H](C)C[C@H]2N(C(C)=O)c1ccc(Cl)cc1
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N(C)C)cc2)c2cc(OCC(N)=O)ccc21
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
105408e964ac437f824a9922364526f556e96df203889ba34fcbafd6bba50fb9
75d17ddc511236e829264b8c8a9fcc5f5e6ae3e810b5d027a6937e62de8e6d83
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
C-C-C(=O)-N(-[C@H]1-C-[C@H](-C)-N(-C(=O)-c2:c:c:c(-F):c:c:2)-[c;H0;D3;+0:1]2:[c:2]:[c:3]:[c:4]:[c:5]:[c;H0;D3;+0:6]:2-1)-c1:c:c:c(-Cl):c:c:1.C-C-O-C(=O)-C-O-c1:c:c:c2:c(:c:1)-[N;H0;D3;+0:7](-[C:8](=[O;D1;H0:9])-[c:10])-[C:11](-[C;D1;H3:12])-[C:13]-[C@H;D3;+0:14]-2-[#7:15](-[c:16])-[C:17](-[C;D1;H3:18])=[O;D1;H0:19]>>[C...
null
[]
null
null
null
null
(±)-Cis-2-[4-[acetyl-(4-chloro-phenyl)-amino]-1-(4-dimethylamino-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-7-yloxy]-acetamide was prepared from (±)-cis-[4-[acetyl-(4-chloro-phenyl)-amino]-1-(4-dimethylamino-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-7-yloxy]-acetic acid ethyl ester, via the same amidation proced...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide.Ester.Ether.Tertiary amide.Tertiary amide.Tertiary amide
Tertiary amide
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCCN2.c1ccc2c(c1)CCC[NH]2
c1ccc2c(c1)CCC[NH]2
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HF
null
null
null
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccc(OCC(N)=O)cc21.CCOC(=O)COc1ccc2c(c1)N(C(=O)c1ccc(N(C)C)cc1)[C@@H](C)C[C@H]2N(C(C)=O)c1ccc(Cl)cc1>>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N(C)C)cc2)c2cc(OCC(N)=O)ccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ea57e68332c645b999b433b378d1e26d
CCOC(=O)COc1ccc2c(c1)N(C(=O)c1ccc(N(C)C)cc1)[C@@H](C)C[C@H]2N(C(C)=O)c1ccc(Cl)cc1>>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N(C)C)cc2)c2cc(OCC(=O)O)ccc21
ClC1=CC=C(C=C1)N([C@@H]1C[C@@H](N(C2=CC=C(C=C12)OCC(=O)O)C(C1=CC=C(C=C1)F)=O)C)C(CC)=O.C(C)OC(COC1=CC=C2[C@@H](C[C@@H](N(C2=C1)C(C1=CC=C(C=C1)N(C)C)=O)C)N(C1=CC=C(C=C1)Cl)C(C)=O)=O>>C(C)(=O)N([C@@H]1C[C@@H](N(C2=CC(=CC=C12)OCC(=O)O)C(C1=CC=C(C=C1)N(C)C)=O)C)C1=CC=C(C=C1)Cl
CC[O:35][C:33]([CH2:32][O:31][c:30]1[cH:29][c:28]2[c:38]([cH:37][cH:36]1)[C@H:12]([N:4]([C:2]([CH3:1])=[O:3])[c:5]1[cH:6][cH:7][c:8]([Cl:9])[cH:10][cH:11]1)[CH2:13][C@H:14]([CH3:15])[N:16]2[C:17](=[O:18])[c:19]1[cH:20][cH:21][c:22]([N:23]([CH3:24])[CH3:25])[cH:26][cH:27]1)=[O:34]>>[CH3:1][C:2](=[O:3])[N:4]([c:5]1[cH:6]...
CCOC(=O)COc1ccc2c(c1)N(C(=O)c1ccc(N(C)C)cc1)[C@@H](C)C[C@H]2N(C(C)=O)c1ccc(Cl)cc1
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N(C)C)cc2)c2cc(OCC(=O)O)ccc21
null
null
null
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
C-C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
null
[]
null
null
null
null
(±)-Cis-[4-[acetyl-(4-chloro-phenyl)-amino]-1-(4-dimethylamino-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-7-yloxy]-acetic acid was prepared from (±)-cis-[4-[acetyl-(4-chloro-phenyl)-amino]-1-(4-dimethylamino-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-7-yloxy]-acetic acid ethyl ester following the saponification p...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
Other
null
null
null
CCOC(=O)COc1ccc2c(c1)N(C(=O)c1ccc(N(C)C)cc1)[C@@H](C)C[C@H]2N(C(C)=O)c1ccc(Cl)cc1>>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(N(C)C)cc2)c2cc(OCC(=O)O)ccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5315f5b4e1174f36bad95a4458c713f7
CCC(=O)OC[C@H]1C[C@@H](N(C(=O)CC)c2ccc(Cl)cc2)c2ccccc2N1C(=O)c1ccc(F)cc1>>CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](CO)N(C(=O)c2ccc(F)cc2)c2ccccc21
ClC1=CC=C(C=C1)N([C@@H]1C[C@@H](N(C2=CC=C(C=C12)OCC(=O)O)C(C1=CC=C(C=C1)F)=O)C)C(CC)=O.ClC1=CC=C(C=C1)N([C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)F)=O)COC(CC)=O)C(CC)=O>>ClC1=CC=C(C=C1)N(C(CC)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)F)=O)CO
CCC(=O)[O:17][CH2:16][C@H:15]1[CH2:14][C@@H:13]([N:5]([C:3]([CH2:2][CH3:1])=[O:4])[c:6]2[cH:7][cH:8][c:9]([Cl:10])[cH:11][cH:12]2)[c:33]2[c:28]([cH:29][cH:30][cH:31][cH:32]2)[N:18]1[C:19](=[O:20])[c:21]1[cH:22][cH:23][c:24]([F:25])[cH:26][cH:27]1>>[CH3:1][CH2:2][C:3](=[O:4])[N:5]([c:6]1[cH:7][cH:8][c:9]([Cl:10])[cH:11]...
CCC(=O)OC[C@H]1C[C@@H](N(C(=O)CC)c2ccc(Cl)cc2)c2ccccc2N1C(=O)c1ccc(F)cc1
CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](CO)N(C(=O)c2ccc(F)cc2)c2ccccc21
null
null
null
Reduction
Hydrolysis or Hydrogenolysis of Carboxylic Esters or Thioesters
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
C-C-C(=O)-[O;H0;D2;+0:1]-[C:2]-[C:3]-[#7:4]>>[#7:4]-[C:3]-[C:2]-[OH;D1;+0:1]
null
[]
null
null
null
null
(±)-Cis-N-(4-chloro-phenyl)-N-[1-(4-fluoro-benzoyl)-2-hydroxymethyl-1,2,3,4-tetrahydro-quinolin-4-yl]-propionamide was prepared from (±)-cis-propionic acid 4-[(4-chloro-phenyl)-propionyl-amino]-1-(4-fluoro-benzoyl)-1,2,3,4-tetrahydro-quinolin-2-ylmethyl ester using the saponification conditions utilized in the synthesi...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HO-
null
null
null
CCC(=O)OC[C@H]1C[C@@H](N(C(=O)CC)c2ccc(Cl)cc2)c2ccccc2N1C(=O)c1ccc(F)cc1>>CCC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](CO)N(C(=O)c2ccc(F)cc2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8401052c572846aba0ef57c8ae4131d5
C[C@@H](COS(C)(=O)=O)NC(=O)OC(C)(C)C.[C-]#N>>C[C@@H](CC#N)NC(=O)OC(C)(C)C
C(C)(C)(C)OC(=O)N[C@H](COS(=O)(=O)C)C.[C-]#N.[Na+]>>C(C)(C)(C)OC(N[C@H](CC#N)C)=O
CS(=O)(=O)O[CH2:3][C@H:2]([CH3:1])[NH:6][C:7](=[O:8])[O:9][C:10]([CH3:11])([CH3:12])[CH3:13].[C-:4]#[N:5]>>[CH3:1][C@@H:2]([CH2:3][C:4]#[N:5])[NH:6][C:7](=[O:8])[O:9][C:10]([CH3:11])([CH3:12])[CH3:13]
C[C@@H](COS(C)(=O)=O)NC(=O)OC(C)(C)C.[C-]#N
C[C@@H](CC#N)NC(=O)OC(C)(C)C
null
[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC.[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC
CN(C=O)C
C-C Coupling
OtherReaction
18f4bbb9c586d5002707644e5539611116bc9c01fc56c5a56ec0d1b0251f5f0b
89d1e6e004e8ba10561e22cfb8893e96c375691951aae8f42243dfb0e0a04eec
null
C-S(=O)(=O)-O-[CH2;D2;+0:1]-[C:2](-[C;D1;H3:3])-[#7:4]-[C:5](=[O;D1;H0:6])-[#8:7]-[C:8](-[C;D1;H3:9])(-[C;D1;H3:10])-[C;D1;H3:11].[C-;H0;D1:12]#[N;D1;H0:13]>>[C;D1;H3:9]-[C:8](-[C;D1;H3:10])(-[C;D1;H3:11])-[#8:7]-[C:5](=[O;D1;H0:6])-[#7:4]-[C:2](-[C;D1;H3:3])-[CH2;D2;+0:1]-[C;H0;D2;+0:12]#[N;D1;H0:13]
null
[]
35
CELSIUS
30
MINUTE
Sodium cyanide (48.92 g, 0.421 mol) was added to dimethylformamide (DMF) (420 mL) and the mixture was stirred at 35° C. for 30 minutes. Tetrabutylammonium bromide (5.22 g, 0.016 mol) was added and the reaction mixture was stirred for an additional 2 h at 35° C. Methanesulfonic acid 2-(S)-tert-butoxycarbonylamino-propyl...
10.6084/m9.figshare.5104873.v1
null
Mesylate
Nitrile
null
null
null
MsOH.HO-
[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC.[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC.CN(C=O)C
35
0.5
C[C@@H](COS(C)(=O)=O)NC(=O)OC(C)(C)C.[C-]#N>[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC.[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC.CN(C=O)C>C[C@@H](CC#N)NC(=O)OC(C)(C)C
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f96025ccacd64add8eb14a33108935cc
C[C@@H](CC#N)Nc1ccccc1.O=S(=O)(O)O>>C[C@@H](CC(N)=O)Nc1ccccc1
C1(=CC=CC=C1)N[C@H](CC#N)C.S(O)(O)(=O)=O>>C1(=CC=CC=C1)N[C@H](CC(=O)N)C
[CH3:1][C@@H:2]([CH2:3][C:4]#[N:5])[NH:7][c:8]1[cH:9][cH:10][cH:11][cH:12][cH:13]1.O=S(=O)(O)[OH:6]>>[CH3:1][C@@H:2]([CH2:3][C:4]([NH2:5])=[O:6])[NH:7][c:8]1[cH:9][cH:10][cH:11][cH:12][cH:13]1
C[C@@H](CC#N)Nc1ccccc1.O=S(=O)(O)O
C[C@@H](CC(N)=O)Nc1ccccc1
null
null
O.C1(=CC=CC=C1)C
Heteroatom Alkylation and Arylation
OtherReaction
1d1793919e847ed86dcb16487e62464531560dbf4782f9a5875bfe7e0477a3ec
d6f9d146e8ef95e62f1a3ab55a7e3b4ceec8856a5f71b6dccd4ad850f945b658
c1ccccc1
O-S(=O)(=O)-[OH;D1;+0:1].[C:2]-[C:3]-[C;H0;D2;+0:4]#[N;H0;D1;+0:5]>>[C:2]-[C:3]-[C;H0;D3;+0:4](-[NH2;D1;+0:5])=[O;H0;D1;+0:1]
null
[]
null
null
0.5
HOUR
To a solution of (S)-3-phenylamino-butyronitrile (6.06 g, 0.0378 mol) in toluene (150 mL) was added a cooled solution of conc. sulfuric acid in H2O (20.12 mL H2SO4/3 mL)—(The ratio of toluene to acid/H2O is very important and should be followed strictly). Stir the biphasic mixture at room temperature for 0.5 h and warm...
10.6084/m9.figshare.5104873.v1
null
Nitrile
Primary amide
null
null
c1ccccc1
Other
O.C1(=CC=CC=C1)C
null
0.5
C[C@@H](CC#N)Nc1ccccc1.O=S(=O)(O)O>O.C1(=CC=CC=C1)C>C[C@@H](CC(N)=O)Nc1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8e1b62f87d064f4ca032f3815c55bcc1
C[C@@H](CC(N)=O)Nc1ccccc1.O=C(Cl)OCc1ccccc1>>C[C@@H](CC(=O)NC(=O)OCc1ccccc1)Nc1ccccc1
CC(C)([O-])C.[Li+].ClC(=O)OCC1=CC=CC=C1.C1(=CC=CC=C1)N[C@H](CC(=O)N)C.CC(C)([O-])C.[Li+]>>C(C1=CC=CC=C1)OC(NC(C[C@H](C)NC1=CC=CC=C1)=O)=O
[CH3:1][C@@H:2]([CH2:3][C:4](=[O:5])[NH2:6])[NH:17][c:18]1[cH:19][cH:20][cH:21][cH:22][cH:23]1.Cl[C:7](=[O:8])[O:9][CH2:10][c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1>>[CH3:1][C@@H:2]([CH2:3][C:4](=[O:5])[NH:6][C:7](=[O:8])[O:9][CH2:10][c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1)[NH:17][c:18]1[cH:19][cH:20][cH:21][cH:2...
C[C@@H](CC(N)=O)Nc1ccccc1.O=C(Cl)OCc1ccccc1
C[C@@H](CC(=O)NC(=O)OCc1ccccc1)Nc1ccccc1
null
null
C1CCOC1
Protection
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
ad1c02b16132fcebf06978727b6e3537fe24971c1b6b51ebd3c2feb87bf80211
e0859034a1689c5b5e475fb10c80f10698b9f2f1df4607fb1088ad38d4759eaf
O=C(CCNc1ccccc1)NC(=O)OCc1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C:4].[C:5]-[C:6](-[NH2;D1;+0:7])=[O;D1;H0:8]>>[C:4]-[#8:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:7]-[C:6](-[C:5])=[O;D1;H0:8]
82
[{"value": 82.0, "product": "C(C1=CC=CC=C1)OC(NC(C[C@H](C)NC1=CC=CC=C1)=O)=O", "details": "PERCENTYIELD", "is_desired": false}]
-10
CELSIUS
null
null
A clean, dry and nitrogen gas purged flask was charged with (S)-3-phenylamino-butyramide (3.25 g, 0.018 mmol) in THF (65 mL) and the mixture was cooled to −10° C. Benzyl chloroformate (3.12 mL, 0.022 mmol) was then added followed by the slow addition of 1.0 M lithium tert-butoxide in THF solution (18 mL). The lithium t...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Ether.Primary amide
Carbamic ester
null
null
c1ccccc1.c1ccccc1
HCl
C1CCOC1
-10
null
C[C@@H](CC(N)=O)Nc1ccccc1.O=C(Cl)OCc1ccccc1>C1CCOC1>C[C@@H](CC(=O)NC(=O)OCc1ccccc1)Nc1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-78c8ee5d4b2b4815abd0fa19411ab3ed
C[C@@H](CC(=O)NC(=O)OCc1ccccc1)Nc1ccccc1>>C[C@H]1C[C@@H](NC(=O)OCc2ccccc2)c2ccccc2N1
C(C1=CC=CC=C1)OC(NC(C[C@H](C)NC1=CC=CC=C1)=O)=O.[BH4-].[Na+]>>C(C1=CC=CC=C1)OC(N[C@@H]1C[C@@H](NC2=CC=CC=C12)C)=O
O=[C:4]([CH2:3][C@H:2]([CH3:1])[NH:22][c:21]1[cH:16][cH:17][cH:18][cH:19][cH:20]1)[NH:5][C:6](=[O:7])[O:8][CH2:9][c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1>>[CH3:1][C@H:2]1[CH2:3][C@@H:4]([NH:5][C:6](=[O:7])[O:8][CH2:9][c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[NH:22]1
C[C@@H](CC(=O)NC(=O)OCc1ccccc1)Nc1ccccc1
C[C@H]1C[C@@H](NC(=O)OCc2ccccc2)c2ccccc2N1
null
null
C(C)O
C-C Coupling
OtherReaction
97f8a9f9c50150a80669192eed2907fad81281a5555d63457333226a47ae997c
d9206c89bc8c29af05511b9e2eee5a949354ced9cafb338d4a7bf26515a328e5
O=C(N[C@@H]1CCNc2ccccc21)OCc1ccccc1
O=[C;H0;D3;+0:1](-[#7:2]-[C:3](-[#8:4])=[O;D1;H0:5])-[C:6]-[C:7]-[#7:8]-[c:9](:[c:10]):[cH;D2;+0:11]:[c:12]:[c:13]>>[#8:4]-[C:3](=[O;D1;H0:5])-[#7:2]-[C@@H;D3;+0:1]1-[C:6]-[C:7]-[#7:8]-[c:9](:[c:10]):[c;H0;D3;+0:11]-1:[c:12]:[c:13]
94
[{"value": 94.0, "product": "C(C1=CC=CC=C1)OC(N[C@@H]1C[C@@H](NC2=CC=CC=C12)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-10
CELSIUS
6
HOUR
A clean, dry flask was charged with (S)-(3-phenylamino-butyryl)-carbamic acid benzyl ester (0.821 g, 2.63 mmol) followed by reagent grade ethanol (20 mL) and cooled to −10° C. Sodium borohydride (0.070 g, 1.84 mmol) was added to the solution in one portion. Nitrogen gas purging is maintained for 5 minutes. A solution o...
10.6084/m9.figshare.5104873.v1
null
Unsubstituted dicarboximide
null
c1ccccc1
c1ccc2c(c1)CCCN2
c1ccccc1.c1ccc2c(c1)CCCN2
Other
C(C)O
-10
6
C[C@@H](CC(=O)NC(=O)OCc1ccccc1)Nc1ccccc1>C(C)O>C[C@H]1C[C@@H](NC(=O)OCc2ccccc2)c2ccccc2N1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-96f5bfdea7b8462ea145cfeac3af6291
CCOC(C)=O.C[C@H]1C[C@@H](N)c2ccccc2N1C(=O)c1ccc(F)cc1.OB(O)c1ccc(Cl)cc1>>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccccc21
C(C)(=O)OCC.N[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(=O)C1=CC=C(C=C1)F)C.ClC1=CC=C(C=C1)B(O)O.N1=CC=CC=C1>>ClC1=CC=C(C=C1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)F)=O)C
CCO[C:2]([CH3:1])=[O:3].[NH2:4][C@@H:12]1[CH2:13][C@H:14]([CH3:15])[N:16]([C:17](=[O:18])[c:19]2[cH:20][cH:21][c:22]([F:23])[cH:24][cH:25]2)[c:26]2[cH:27][cH:28][cH:29][cH:30][c:31]21.OB(O)[c:5]1[cH:6][cH:7][c:8]([Cl:9])[cH:10][cH:11]1>>[CH3:1][C:2](=[O:3])[N:4]([c:5]1[cH:6][cH:7][c:8]([Cl:9])[cH:10][cH:11]1)[C@@H:12]1...
CCOC(C)=O.C[C@H]1C[C@@H](N)c2ccccc2N1C(=O)c1ccc(F)cc1.OB(O)c1ccc(Cl)cc1
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccccc21
null
C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-]
CN(C)C=O
Acylation
OtherReaction
d5b79df0bcad37b68666465f98bdbf09561dfcc3b18a2acc5b3be323501cddff
d21a41b88b3a6857658a80208e904dc455b890b23aaf7d742d8a593a93afbd98
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
C-C-O-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].O-B(-O)-[c;H0;D3;+0:4](:[c:5]:[c:6]):[c:7]:[c:8].[C:9]-[C:10](-[NH2;D1;+0:11])-[c:12]>>[C:9]-[C:10](-[N;H0;D3;+0:11](-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3])-[c;H0;D3;+0:4](:[c:5]:[c:6]):[c:7]:[c:8])-[c:12]
18
[{"value": 18.0, "product": "ClC1=CC=C(C=C1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)F)=O)C", "details": "PERCENTYIELD", "is_desired": false}]
60
CELSIUS
1
HOUR
To a solution of (2S,4R)-(4-amino-2-methyl-3,4-dihydro-2H-quinolin-1-yl)-(4-fluoro-phenyl)-methanone (1.0 g, 3.5 mmol) in DMF (20 mL, dry) was added 4-chlorophenylboronic acid (1.1 g, 7.0 mmol), pyridine (850 uL, 10.5 mmol) and copper(II)acetate (1.27 g, 7.0 mmol). The heterogeneous green mixture was stirred open to ai...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine.Boronic acid
Tertiary amide
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HO-.B
C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-].CN(C)C=O
60
1
CCOC(C)=O.C[C@H]1C[C@@H](N)c2ccccc2N1C(=O)c1ccc(F)cc1.OB(O)c1ccc(Cl)cc1>C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-].CN(C)C=O>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b0470e7758a04de497501c90395f8ef7
CC(=O)Cl.C[C@H]1C[C@@H](Nc2ccc(Cl)cc2)c2ccccc2N1C(=O)c1ccc(F)cc1>>CC(=O)N(c1ccc(Cl)cc1)C1CC(C)N(C(=O)c2ccc(F)cc2)c2ccccc21
C(C)(=O)Cl.ClC1=CC=C(C=C1)N[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(=O)C1=CC=C(C=C1)F)C.C(C)(C)N(CC)C(C)C>>ClC1=CC=C(C=C1)N(C(C)=O)C1CC(N(C2=CC=CC=C12)C(C1=CC=C(C=C1)F)=O)C
Cl[C:2]([CH3:1])=[O:3].[NH:4]([c:5]1[cH:6][cH:7][c:8]([Cl:9])[cH:10][cH:11]1)[C@@H:12]1[CH2:13][C@H:14]([CH3:15])[N:16]([C:17](=[O:18])[c:19]2[cH:20][cH:21][c:22]([F:23])[cH:24][cH:25]2)[c:26]2[cH:27][cH:28][cH:29][cH:30][c:31]21>>[CH3:1][C:2](=[O:3])[N:4]([c:5]1[cH:6][cH:7][c:8]([Cl:9])[cH:10][cH:11]1)[CH:12]1[CH2:13]...
CC(=O)Cl.C[C@H]1C[C@@H](Nc2ccc(Cl)cc2)c2ccccc2N1C(=O)c1ccc(F)cc1
CC(=O)N(c1ccc(Cl)cc1)C1CC(C)N(C(=O)c2ccc(F)cc2)c2ccccc21
null
null
C(Cl)Cl
Acylation
N-alkylation of secondary amines with alkyl halides
b92e0bfd3d683c1f2a209adfe70a67ad7cb0d87749eb59e8fe0cf1689bc291e0
96cb0a2fed10552c5770a45a2d6523b47ac3e38928b4a9c698d8577451182dcd
O=C(c1ccccc1)N1CCC(Nc2ccccc2)c2ccccc21
Cl-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[c:4]:[c:5](-[NH;D2;+0:6]-[C@@H;D3;+0:7]1-[C:8]-[C:9]-[#7:10]-[c:11]:[c:12]-1:[c:13]):[c:14]>>[C;D1;H3:2]-[C;H0;D3;+0:1](=[O;D1;H0:3])-[N;H0;D3;+0:6](-[CH;D3;+0:7]1-[C:8]-[C:9]-[#7:10]-[c:11]:[c:12]-1:[c:13])-[c:5](:[c:4]):[c:14]
72
[{"value": 71.0, "product": "ClC1=CC=C(C=C1)N(C(C)=O)C1CC(N(C2=CC=CC=C12)C(C1=CC=C(C=C1)F)=O)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 72.0, "product": "ClC1=CC=C(C=C1)N(C(C)=O)C1CC(N(C2=CC=CC=C12)C(C1=CC=C(C=C1)F)=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
To a solution of (2S,4R)-[4-(4-chloro-phenylamino)-2-methyl-3,4-dihydro-2H-quinolin-1-yl]-(4-fluoro-phenyl)-methanone (250 mg, 0.636 mmol) in methylene chloride (5 mL) was added diisopropylethylamine (120 uL, 0.70 mmol) followed by acetyl chloride (90 uL, 1.27 mmol). The mixture was stirred at rt 4 h. The mixture was c...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Secondary amine
Tertiary amide
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HCl
C(Cl)Cl
null
4
CC(=O)Cl.C[C@H]1C[C@@H](Nc2ccc(Cl)cc2)c2ccccc2N1C(=O)c1ccc(F)cc1>C(Cl)Cl>CC(=O)N(c1ccc(Cl)cc1)C1CC(C)N(C(=O)c2ccc(F)cc2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-bae6b406dd2747c996157f43a18e49cc
CCC(=O)N(c1ccc(Cl)cc1)C1CC(C)N(C(=O)c2ccc(OCCCC(=O)O)cc2)c2ccccc21>>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(OCCCC(=O)O)cc2)c2ccccc21
FC1=CC=C(C(=O)Cl)C=C1.ClC1=CC=C(C=C1)N(C1CC(N(C2=CC=CC=C12)C(=O)C1=CC=C(OCCCC(=O)O)C=C1)C)C(CC)=O>>C(C)(=O)N([C@@H]1C[C@@H](N(C2=CC=CC=C12)C(=O)C1=CC=C(OCCCC(=O)O)C=C1)C)C1=CC=C(C=C1)Cl
C[CH2:1][C:2](=[O:3])[N:4]([c:5]1[cH:6][cH:7][c:8]([Cl:9])[cH:10][cH:11]1)[CH:12]1[CH2:13][CH:14]([CH3:15])[N:16]([C:17](=[O:18])[c:19]2[cH:20][cH:21][c:22]([O:23][CH2:24][CH2:25][CH2:26][C:27](=[O:28])[OH:29])[cH:30][cH:31]2)[c:32]2[cH:33][cH:34][cH:35][cH:36][c:37]21>>[CH3:1][C:2](=[O:3])[N:4]([c:5]1[cH:6][cH:7][c:8]...
CCC(=O)N(c1ccc(Cl)cc1)C1CC(C)N(C(=O)c2ccc(OCCCC(=O)O)cc2)c2ccccc21
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(OCCCC(=O)O)cc2)c2ccccc21
null
null
null
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
C-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#7:4](-[C:5])-[c:6]>>[C:5]-[#7:4](-[c:6])-[C:2](-[CH3;D1;+0:1])=[O;D1;H0:3]
null
[]
null
null
null
null
(2S,4R)-4-(4-{4-[Acetyl-(4-chloro-phenyl)-amino]-2-methyl-3,4-dihydro-2H-quinoline-1-carbonyl}-phenoxy)-butyric acid was prepared was made following general procedure C, substituting 4-methoxybenzoyl chloride for 4-fluorobenzoyl chloride. Further elaboration to the acid was done following the same procedure as describe...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
Other
null
null
null
CCC(=O)N(c1ccc(Cl)cc1)C1CC(C)N(C(=O)c2ccc(OCCCC(=O)O)cc2)c2ccccc21>>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(OCCCC(=O)O)cc2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-aed14fa894c74c0081111ee7611cf940
BrCc1ccncc1.COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)cc1>>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(OCc3ccncc3)cc2)c2ccccc21
C(C)O.[H-].[Na+].ClC1=CC=C(C=C1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C.BrCC1=CC=NC=C1>>ClC1=CC=C(C=C1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OCC1=CC=NC=C1)=O)C
BrC[c:25]1[cH:26][cH:27][n:28][cH:29][cH:30]1.[CH3:1][C:2](=[O:3])[N:4]([c:5]1[cH:6][cH:7][c:8]([Cl:9])[cH:10][cH:11]1)[C@@H:12]1[CH2:13][C@H:14]([CH3:15])[N:16]([C:17](=[O:18])[c:19]2[cH:20][cH:21][c:22]([O:23][CH3:24])[cH:31][cH:32]2)[c:33]2[cH:34][cH:35][cH:36][cH:37][c:38]21>>[CH3:1][C:2](=[O:3])[N:4]([c:5]1[cH:6][...
BrCc1ccncc1.COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)cc1
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(OCc3ccncc3)cc2)c2ccccc21
null
null
CN(C)C=O
C-C Coupling
OtherReaction
9282e47746c7b9fca3e9abca83ead5e293ef27502e62bd81a3cdbf12d8372825
2c1c1647472d7e3cff37f0f3aad955b760f0ad2f8b7aa7e7825b1c0344bab3bb
O=C(c1ccc(OCc2ccncc2)cc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
Br-C-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[#7;a:4]:[c:5]:[c:6]:1.[CH3;D1;+0:7]-[#8:8]-[c:9]>>[c:9]-[#8:8]-[CH2;D2;+0:7]-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[#7;a:4]:[c:5]:[c:6]:1
null
[]
null
null
30
MINUTE
The phenol was dissolved in DMF (5 mL) at room temperature. Sodium hydride (60% in oil) was added and the mixture allowed to stir 30 min. 4-Bromomethyl-pyridine was added and the reaction was allowed to stir over night. Ethanol was added and the reaction was concentrated in vacuo. The residue was partitioned between et...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ether
Ether
c1ccncc1
c1ccncc1
c1ccccc1.c1ccccc1.c1ccncc1.c1ccc2c(c1)CCC[NH]2
HBr
CN(C)C=O
null
0.5
BrCc1ccncc1.COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)cc1>CN(C)C=O>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(OCc3ccncc3)cc2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-52c7f3ae7670408d9755bccd1a1bed37
CCC(=O)N(c1ccccc1)C1CC(C)N(C(=O)c2ccc(O)cc2)c2ccccc21.O=C(Cl)c1ccc(F)cc1>>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(O)cc2)c2ccccc21
FC1=CC=C(C(=O)Cl)C=C1.C1(=CC=CC=C1)O.OC1=CC=C(C(=O)N2C(CC(C3=CC=CC=C23)N(C(CC)=O)C2=CC=CC=C2)C)C=C1>>ClC1=CC=C(C=C1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)O)=O)C
C[CH2:1][C:2](=[O:3])[N:4]([c:5]1[cH:6][cH:7][cH:8][cH:10][cH:11]1)[CH:12]1[CH2:13][CH:14]([CH3:15])[N:16]([C:17](=[O:18])[c:19]2[cH:20][cH:21][c:22]([OH:23])[cH:24][cH:25]2)[c:26]2[cH:27][cH:28][cH:29][cH:30][c:31]21.O=C(c1ccc(F)cc1)[Cl:9]>>[CH3:1][C:2](=[O:3])[N:4]([c:5]1[cH:6][cH:7][c:8]([Cl:9])[cH:10][cH:11]1)[C@@H...
CCC(=O)N(c1ccccc1)C1CC(C)N(C(=O)c2ccc(O)cc2)c2ccccc21.O=C(Cl)c1ccc(F)cc1
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(O)cc2)c2ccccc21
null
null
null
Functional Group Interconversion
OtherReaction
91851756c52985d744aa40d2d8891afc4047f94a007ece2d25e4ce655531031f
dceb12a388b2a36b2ea72c892c8b5aa97f970ff7bfb3715e72f5be3e6fa67402
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
C-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#7:4](-[C:5])-[c:6]1:[c:7]:[c:8]:[cH;D2;+0:9]:[c:10]:[c:11]:1.F-c1:c:c:c(-C(=O)-[Cl;H0;D1;+0:12]):c:c:1>>[C:5]-[#7:4](-[C:2](-[CH3;D1;+0:1])=[O;D1;H0:3])-[c:6]1:[c:7]:[c:8]:[c;H0;D3;+0:9](-[Cl;H0;D1;+0:12]):[c:10]:[c:11]:1
null
[]
null
null
null
null
(2S,4R)-N-(4-Chloro-phenyl)-N-[1-(4-hydroxy-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-acetamide was prepared was made following general procedure C, substituting 3-methoxybenzoyl chloride for 4-fluorobenzoyl chloride. Further elaboration to the phenol was done following the same procedure as described for (±)...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Aromatic halide
Aromatic halide
c1ccccc1.c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HF
null
null
null
CCC(=O)N(c1ccccc1)C1CC(C)N(C(=O)c2ccc(O)cc2)c2ccccc21.O=C(Cl)c1ccc(F)cc1>>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(O)cc2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-258b5262bc1b4c1995a55ec514facab1
CC(=O)c1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)cc1>>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(C(C)(C)O)cc2)c2ccccc21
C[Mg]Br.C(C)(=O)C1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N(C(C)=O)C2=CC=C(C=C2)Cl)C)C=C1.C(C)(=O)C1=CC=C(C(=O)N2[C@H](C[C@H](C3=CC=CC=C23)N(C(C)=O)C2=CC=C(C=C2)Cl)C)C=C1.[Cl-].[NH4+]>>ClC1=CC=C(C=C1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)C(C)(C)O)=O)C
[CH3:1][C:2](=[O:3])[N:4]([c:5]1[cH:6][cH:7][c:8]([Cl:9])[cH:10][cH:11]1)[C@@H:12]1[CH2:13][C@H:14]([CH3:15])[N:16]([C:17](=[O:18])[c:19]2[cH:20][cH:21][c:22]([C:23]([CH3:24])=[O:26])[cH:27][cH:28]2)[c:29]2[cH:30][cH:31][cH:32][cH:33][c:34]21>>[CH3:1][C:2](=[O:3])[N:4]([c:5]1[cH:6][cH:7][c:8]([Cl:9])[cH:10][cH:11]1)[C@...
CC(=O)c1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)cc1
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(C(C)(C)O)cc2)c2ccccc21
null
null
C1CCOC1
Miscellaneous
OtherReaction
7e61014f084ef66fe8691c8f1abaf493e11079effe9d87ae329e041d937b8b3a
8811b4d793f7cfa9f0f1f47a008648edabb54f371f76dfa680dd5b2e1564c6c5
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
[C;D1;H3:1]-[C;H0;D3;+0:2](=[O;H0;D1;+0:3])-[c:4](:[c:5]):[c:6]>>[C;D1;H3:1]-[C;H0;D4;+0:2](-[C;D1;H3:7])(-[OH;D1;+0:3])-[c:4](:[c:5]):[c:6]
24
[{"value": 24.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
0
CELSIUS
2
HOUR
(2S,4R)-N-(4-Chloro-phenyl)-N-{1-[4-(1-hydroxy-1-methyl-ethyl)-benzoyl]-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl}-acetamide was prepared from (2S,4R)-N-[1-(4-acetyl-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-N-(4-chloro-phenyl)-acetamide. (2S,4R)-N-[1-(4-Acetyl-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-...
10.6084/m9.figshare.5104873.v1
null
Ketone
Tertiary alcohol
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
Other
C1CCOC1
0
2
CC(=O)c1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)cc1>C1CCOC1>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(C(C)(C)O)cc2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4f0a98b5259a41a8ba3de6adcfa42b29
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(C=CC(=O)O)cc2)c2ccccc21>>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(CCC(=O)O)cc2)c2ccccc21
C(C)(=O)N([C@@H]1C[C@@H](N(C2=CC=CC=C12)C(=O)C1=CC=C(C=C1)C=CC(=O)O)C)C1=CC=C(C=C1)Cl.C(C)(=O)N([C@@H]1C[C@@H](N(C2=CC=CC=C12)C(=O)C1=CC=C(C=C1)C=CC(=O)O)C)C1=CC=C(C=C1)Cl>>C(C)(=O)N([C@@H]1C[C@@H](N(C2=CC=CC=C12)C(=O)C1=CC=C(C=C1)CCC(=O)O)C)C1=CC=C(C=C1)Cl
[CH3:1][C:2](=[O:3])[N:4]([c:5]1[cH:6][cH:7][c:8]([Cl:9])[cH:10][cH:11]1)[C@@H:12]1[CH2:13][C@H:14]([CH3:15])[N:16]([C:17](=[O:18])[c:19]2[cH:20][cH:21][c:22]([CH:23]=[CH:24][C:25](=[O:26])[OH:27])[cH:28][cH:29]2)[c:30]2[cH:31][cH:32][cH:33][cH:34][c:35]21>>[CH3:1][C:2](=[O:3])[N:4]([c:5]1[cH:6][cH:7][c:8]([Cl:9])[cH:1...
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(C=CC(=O)O)cc2)c2ccccc21
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(CCC(=O)O)cc2)c2ccccc21
null
C(Cl)Cl.[Pd]
CCO
Reduction
Hydrogenation (double to single)
0bc3968b35f0839c230afb4215314da278abd4e1f10e42ec3012c5512de49ea5
312e9350dcad67590617294c0eb017edf0b9fbfe6133c06a3f393b871a889092
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
[O;D1;H0:1]=[C:2](-[O;D1;H1:3])-[CH;D2;+0:4]=[CH;D2;+0:5]-[c:6](:[c:7]):[c:8]>>[O;D1;H0:1]=[C:2](-[O;D1;H1:3])-[CH2;D2;+0:4]-[CH2;D2;+0:5]-[c:6](:[c:7]):[c:8]
99
[{"value": 99.0, "product": "C(C)(=O)N([C@@H]1C[C@@H](N(C2=CC=CC=C12)C(=O)C1=CC=C(C=C1)CCC(=O)O)C)C1=CC=C(C=C1)Cl", "details": "PERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
(2S,4R)-3-(4-{4-[Acetyl-(4-chloro-phenyl)-amino]-2-methyl-3,4-dihydro-2H-quinoline-1-carbonyl}-phenyl)-propionic acid was prepared from (2S,4R)-3-(4-{4-[acetyl-(4-chloro-phenyl)-amino]-2-methyl-3,4-dihydro-2H-quinoline-1-carbonyl}-phenyl)-acrylic acid. A solution of (2S,4R)-3-(4-{4-[acetyl-(4-chloro-phenyl)-amino]-2-me...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
null
C(Cl)Cl.[Pd].CCO
null
1
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(C=CC(=O)O)cc2)c2ccccc21>C(Cl)Cl.[Pd].CCO>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(CCC(=O)O)cc2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6265fcbda6b84c8bb5e65fe278b1e988
COC(=O)C=Cc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)cc1>>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(C=CC(=O)O)cc2)c2ccccc21
FC1=CC=C(C(=O)Cl)C=C1.COC(C=CC1=CC=C(C=C1)C(=O)N1[C@H](C[C@H](C2=CC=CC=C12)N(C1=CC=C(C=C1)Cl)C(C)=O)C)=O.[Li+].[OH-]>>C(C)(=O)N([C@@H]1C[C@@H](N(C2=CC=CC=C12)C(=O)C1=CC=C(C=C1)C=CC(=O)O)C)C1=CC=C(C=C1)Cl
C[O:27][C:25]([CH:24]=[CH:23][c:22]1[cH:21][cH:20][c:19]([C:17]([N:16]2[C@@H:14]([CH3:15])[CH2:13][C@@H:12]([N:4]([C:2]([CH3:1])=[O:3])[c:5]3[cH:6][cH:7][c:8]([Cl:9])[cH:10][cH:11]3)[c:35]3[c:30]2[cH:31][cH:32][cH:33][cH:34]3)=[O:18])[cH:29][cH:28]1)=[O:26]>>[CH3:1][C:2](=[O:3])[N:4]([c:5]1[cH:6][cH:7][c:8]([Cl:9])[cH:...
COC(=O)C=Cc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)cc1
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(C=CC(=O)O)cc2)c2ccccc21
null
null
C1CCOC1.CO
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[C:4]=[C:5]-[c:6]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[C:4]=[C:5]-[c:6]
99
[{"value": 99.0, "product": "C(C)(=O)N([C@@H]1C[C@@H](N(C2=CC=CC=C12)C(=O)C1=CC=C(C=C1)C=CC(=O)O)C)C1=CC=C(C=C1)Cl", "details": "PERCENTYIELD", "is_desired": false}, {"value": 94.1, "product": "C(C)(=O)N([C@@H]1C[C@@H](N(C2=CC=CC=C12)C(=O)C1=CC=C(C=C1)C=CC(=O)O)C)C1=CC=C(C=C1)Cl", "details": "CALCULATEDPERCENTYIELD", "...
null
null
null
null
(2S,4R)-3-(4-{4-[Acetyl-(4-chloro-phenyl)-amino]-2-methyl-3,4-dihydro-2H-quinoline-1-carbonyl}-phenyl)-acrylic acid was prepared following general procedure C, substituting 3-(4-chlorocarbonyl-phenyl)-acrylic acid methyl ester for 4-fluorobenzoyl chloride. The ester was hydrolyzed as follows. To a solution of (2S,4R)-3...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
Other
C1CCOC1.CO
null
null
COC(=O)C=Cc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(Cl)cc3)C[C@@H]2C)cc1>C1CCOC1.CO>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(C=CC(=O)O)cc2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e71a2a67cf1645d3b3e373d992e9d838
COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3cccc(C#N)c3)C[C@@H]2C)cc1.O=C(Cl)c1ccc(F)cc1>>COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3cccc(CN)c3)C[C@@H]2C)cc1
C(#N)C=1C=C(C=CC1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C.C(#N)C=1C=C(C=CC1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C.[BH4-].[Na+].FC1=CC=C(C(=O)Cl)C=C1>>C(#N)C=1C=C(C=CC1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C.NCC=1C=C(C=CC1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=...
C(c1[cH:57][cH:56][cH:55][c:54]([N:50]([C@H:49]2[c:48]3[c:43]([cH:44][cH:45][cH:46][cH:47]3)[N:42]([C:40]([c:39]3[cH:38][cH:37][c:36]([O:35][CH3:34])[cH:66][cH:65]3)=[O:41])[C@@H:63]([CH3:64])[CH2:62]2)[C:51]([CH3:52])=[O:53])[cH:61]1)#[N:60].O=[C:59](Cl)[c:58]1ccc(F)cc1>>[CH3:34][O:35][c:36]1[cH:37][cH:38][c:39]([C:40...
COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3cccc(C#N)c3)C[C@@H]2C)cc1.O=C(Cl)c1ccc(F)cc1
COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3cccc(CN)c3)C[C@@H]2C)cc1
null
[Co](Cl)Cl
C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
b216327a21510acfef04d829ba4e934585cd7a21b66b2c5734a3dc14ea5d17bd
30938830d4a4929ce2292ebee3b8ab24d74bb12b8b4fc72ec5814d3becc1c450
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
Cl-[C;H0;D3;+0:1](=O)-[c;H0;D3;+0:2]1:c:c:c(-F):c:c:1.[C;D1;H3:3]-[C:4](=[O;D1;H0:5])-[#7:6]-[c:7]1:[c:8]:[c:9]:[cH;D2;+0:10]:c(-C#[N;H0;D1;+0:11]):[cH;D2;+0:12]:1>>[C;D1;H3:3]-[C:4](=[O;D1;H0:5])-[#7:6]-[c:7]1:[c:8]:[c:9]:[cH;D2;+0:10]:[c;H0;D3;+0:2](-[CH2;D2;+0:1]-[NH2;D1;+0:11]):[cH;D2;+0:12]:1
10
[{"value": 10.0, "product": "NCC=1C=C(C=CC1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
(2S,4R)-N-(3-Aminomethyl-phenyl)-N-[1-(4-methoxy-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-acetamide was prepared from (2S,4R)-N-(3-cyano-phenyl)-N-[1-(4-methoxy-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-acetamide. (2S,4R)-N-(3-cyano-phenyl)-N-[1-(4-methoxy-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quino...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Aromatic halide.Nitrile
Primary amine
c1ccccc1.c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
Other
[Co](Cl)Cl.C(C)O
null
0.5
COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3cccc(C#N)c3)C[C@@H]2C)cc1.O=C(Cl)c1ccc(F)cc1>[Co](Cl)Cl.C(C)O>COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3cccc(CN)c3)C[C@@H]2C)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e81126a2972b4b7b9b10dc3e1743a4d9
CN(C)c1ccccc1-c1ccccc1P(C1CCCCC1)C1CCCCC1.COC(=O)COc1ccc(Br)cc1.COc1ccc(C(=O)N2c3ccccc3[C@H](N)C[C@@H]2C)cc1>>COC(=O)COc1ccc(N(C(C)=O)C2CC(C)N(C(=O)c3ccc(OC)cc3)c3ccccc32)cc1
N[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(=O)C1=CC=C(C=C1)OC)C.COC(COC1=CC=C(C=C1)Br)=O.C1(CCCCC1)P(C1=C(C=CC=C1)C1=C(C=CC=C1)N(C)C)C1CCCCC1.C([O-])([O-])=O.[Cs+].[Cs+]>>COC(COC1=CC=C(C=C1)N(C1CC(N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C)C(C)=O)=O
CN(c1ccccc1-c1ccccc1P(C1CCCCC1)C1CCCCC1)[CH3:13].Br[c:10]1[cH:9][cH:8][c:7]([O:6][CH2:5][C:3]([O:2][CH3:1])=[O:4])[cH:37][cH:36]1.[NH2:11][C@@H:15]1[CH2:16][C@H:17]([CH3:18])[N:19]([C:20](=[O:21])[c:22]2[cH:23][cH:24][c:25]([O:26][CH3:27])[cH:28][cH:29]2)[c:30]2[cH:31][cH:32][cH:33][cH:34][c:35]21>>[CH3:1][O:2][C:3](=[...
CN(C)c1ccccc1-c1ccccc1P(C1CCCCC1)C1CCCCC1.COC(=O)COc1ccc(Br)cc1.COc1ccc(C(=O)N2c3ccccc3[C@H](N)C[C@@H]2C)cc1
COC(=O)COc1ccc(N(C(C)=O)C2CC(C)N(C(=O)c3ccc(OC)cc3)c3ccccc32)cc1
null
C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd]
null
Acylation
OtherReaction
abd1394f6614c07911880959c73166f1d80d55d529360e81d9eb77f2886869ee
a542a495d08c4dba580c830cb345c6604739448dfac19f34f92ca5bf1236ec6f
O=C(c1ccccc1)N1CCC(Nc2ccccc2)c2ccccc21
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].C-N(-[CH3;D1;+0:6])-c1:c:c:c:c:c:1-c1:c:c:c:c:c:1-P(-C1-C-C-C-C-C-1)-C1-C-C-C-C-C-1.[NH2;D1;+0:7]-[C@@H;D3;+0:8]1-[C:9]-[C:10]-[#7:11]-[c:12]:[c:13]-1:[c:14]>>[CH3;D1;+0:6]-[C:15](=[O;D1;H0:16])-[N;H0;D3;+0:7](-[CH;D3;+0:8]1-[C:9]-[C:10]-[#7:11]-[c:12]:[c:13]-1:[c:14])-[c;H0;...
368.1
[{"value": 24.0, "product": "COC(COC1=CC=C(C=C1)N(C1CC(N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C)C(C)=O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 368.1, "product": "COC(COC1=CC=C(C=C1)N(C1CC(N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C)C(C)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
24
HOUR
(2S,4R)-(4-Amino-2-methyl-3,4-dihydro-2H-quinolin-1-yl)-(4-methoxyphenyl)-methanone (100 mg, 0.34 mmol), methyl-2-(4-bromophenoxy)-acetate (91 mg, 0.37 mmol), Pd2(dba)3 (17 mg, 0.02 mmol), 2-dicyclohexylphosphino-2′-(N,N-dimethylamino)biphenyl (8 mg, 0.00002 mol) and cesium carbonate (0.163 g, 0.0005 mol) were taken in...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine.Tertiary amine
Tertiary amide
c1ccccc1.c1ccccc1.C1CCCCC1.C1CCCCC1.c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HBr
C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd]
100
24
CN(C)c1ccccc1-c1ccccc1P(C1CCCCC1)C1CCCCC1.COC(=O)COc1ccc(Br)cc1.COc1ccc(C(=O)N2c3ccccc3[C@H](N)C[C@@H]2C)cc1>C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.C=1C=CC(=CC1)/C=C/C(=O)/C=C/C2=CC=CC=C2.[Pd].[Pd]>COC(=O)COc1ccc(N(C(C)=O)C2CC(C)N(C(=O)c3ccc(OC)cc3)c3ccccc32)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d44b3b37fcab42e6b0f744bd0f650667
COC(=O)COc1ccc(N(C(C)=O)[C@@H]2C[C@H](C)N(C(=O)c3ccc(OC)cc3)c3ccccc32)cc1>>COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(OCC(=O)O)cc3)C[C@@H]2C)cc1
Cl.COC(COC1=CC=C(C=C1)N([C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C)C(C)=O)=O.[OH-].[Na+]>>C(C)(=O)N(C1=CC=C(OCC(=O)O)C=C1)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C
C[O:29][C:27]([CH2:26][O:25][c:24]1[cH:23][cH:22][c:21]([N:17]([C@H:16]2[c:15]3[c:10]([cH:11][cH:12][cH:13][cH:14]3)[N:9]([C:7]([c:6]3[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:36][cH:35]3)=[O:8])[C@@H:33]([CH3:34])[CH2:32]2)[C:18]([CH3:19])=[O:20])[cH:31][cH:30]1)=[O:28]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([C:7](=[O:8])[N:9]...
COC(=O)COc1ccc(N(C(C)=O)[C@@H]2C[C@H](C)N(C(=O)c3ccc(OC)cc3)c3ccccc32)cc1
COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(OCC(=O)O)cc3)C[C@@H]2C)cc1
null
null
CO
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
89
[{"value": 89.0, "product": "C(C)(=O)N(C1=CC=C(OCC(=O)O)C=C1)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 88.7, "product": "C(C)(=O)N(C1=CC=C(OCC(=O)O)C=C1)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C", "details": "CALCULATEDPERCENTYIELD", "is...
null
null
18
HOUR
(2S,4R)-(4-{Acetyl-[1-(4-methoxybenzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-amino}-phenoxy)-acetic acid was prepared from (2S,4R)-(4-{acetyl-[1-(4-methoxybenzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-amino}-phenoxy)-acetic acid methyl ester (15 mg, 0.03 mmol). The methyl ester was dissolved in methanol (1...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
Other
CO
null
18
COC(=O)COc1ccc(N(C(C)=O)[C@@H]2C[C@H](C)N(C(=O)c3ccc(OC)cc3)c3ccccc32)cc1>CO>COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(OCC(=O)O)cc3)C[C@@H]2C)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-696adee031184bf4b13a8623daac27c8
COC(=O)C(C)(C)c1ccc(N(C(C)=O)C2CC(C)N(C(=O)c3ccc(OC)cc3)c3ccccc32)cc1>>COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(C(C)(C)C(=O)O)cc3)C[C@@H]2C)cc1
COC(COC1=CC=C(C=C1)Br)=O.COC(C(C)(C)C1=CC=C(C=C1)N(C1CC(N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C)C(C)=O)=O.C(C)(=O)N(C1=CC=C(OCC(=O)O)C=C1)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C>>C(C)(=O)N(C1=CC=C(C=C1)C(C(=O)O)(C)C)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C
C[O:30][C:28]([C:25]([c:24]1[cH:23][cH:22][c:21]([N:17]([CH:16]2[c:15]3[c:10]([cH:11][cH:12][cH:13][cH:14]3)[N:9]([C:7]([c:6]3[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:37][cH:36]3)=[O:8])[CH:34]([CH3:35])[CH2:33]2)[C:18]([CH3:19])=[O:20])[cH:32][cH:31]1)([CH3:26])[CH3:27])=[O:29]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([C:7](=[O...
COC(=O)C(C)(C)c1ccc(N(C(C)=O)C2CC(C)N(C(=O)c3ccc(OC)cc3)c3ccccc32)cc1
COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(C(C)(C)C(=O)O)cc3)C[C@@H]2C)cc1
null
null
null
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
null
[]
null
null
null
null
(2S,4R)-2-(4-{Acetyl-[1-(4-methoxy-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-amino}-phenyl)-2-methyl-propionic acid was prepared via saponification of 2-(4-{acetyl-[1-(4-methoxy-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]amino}-phenyl)-2-methyl-propionic acid methyl ester, as described in the synthesi...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
Other
null
null
null
COC(=O)C(C)(C)c1ccc(N(C(C)=O)C2CC(C)N(C(=O)c3ccc(OC)cc3)c3ccccc32)cc1>>COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(C(C)(C)C(=O)O)cc3)C[C@@H]2C)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1170fa84bc654bc192bedb726b3595fa
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(CCC(=O)O)cc2)c2ccccc21.COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(Br)cc3)C[C@@H]2C)cc1>>COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(CCC(=O)O)cc3)C[C@@H]2C)cc1
ClC1=CC=C(C=C1)N(C1CC(N(C2=CC=C(C=C12)C=CC(=O)O)C(C1=CC=C(C=C1)F)=O)C)C(CC)=O.C(C)(=O)N([C@@H]1C[C@@H](N(C2=CC=CC=C12)C(=O)C1=CC=C(C=C1)CCC(=O)O)C)C1=CC=C(C=C1)Cl.BrC1=CC=C(C=C1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C.BrC1=CC=C(C=C1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C.C(C...
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc([CH2:25][CH2:26][C:27](=[O:28])[OH:29])cc2)c2ccccc21.Br[c:24]1[cH:23][cH:22][c:21]([N:17]([C@H:16]2[c:15]3[c:10]([cH:11][cH:12][cH:13][cH:14]3)[N:9]([C:7]([c:6]3[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:36][cH:35]3)=[O:8])[C@@H:33]([CH3:34])[CH2:32]2)[C:18]([CH3:19])=[O:20])[c...
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(CCC(=O)O)cc2)c2ccccc21.COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(Br)cc3)C[C@@H]2C)cc1
COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(CCC(=O)O)cc3)C[C@@H]2C)cc1
null
null
null
C-C Coupling
OtherReaction
f5c50fc2c2386f32cfff3e799dacf9c36794fb59889488b2f3e337b8f2d1b5e2
421f33baaa7a49fff154f8252433aba113450bc8a477e8366c5f908df290b3b2
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].C-C(=O)-N(-[C@H]1-C-[C@H](-C)-N(-C(=O)-c2:c:c:c(-[CH2;D2;+0:6]-[C:7]-[C:8](=[O;D1;H0:9])-[O;D1;H1:10]):c:c:2)-c2:c:c:c:c:c:2-1)-c1:c:c:c(-Cl):c:c:1>>[O;D1;H0:9]=[C:8](-[O;D1;H1:10])-[C:7]-[CH2;D2;+0:6]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
null
[]
null
null
null
null
(2S,4R)-3-(4-{Acetyl-[1-(4-methoxy-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-amino}-phenyl)-propionic acid was prepared from (2S,4R)-N-(4-bromo-phenyl)-N-[1-(4-methoxy-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-acetamide. (2S,4R)-N-(4-Bromo-phenyl)-N-[1-(4-methoxy-benzoyl)-2-methyl-1,2,3,4-tetrahydro...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide.Tertiary amide.Tertiary amide
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCCN2.c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HCl.Br-
null
null
null
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(CCC(=O)O)cc2)c2ccccc21.COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(Br)cc3)C[C@@H]2C)cc1>>COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(CCC(=O)O)cc3)C[C@@H]2C)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-35c49c134b2142b981b72b68aabeb3d5
COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(CCC(=O)O)cc3)C[C@@H]2C)cc1.[NH4+]>>COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(CCC(N)=O)cc3)C[C@@H]2C)cc1
C(C)(=O)N(C1=CC=C(C=C1)CCC(=O)O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C.C(C)(=O)N(C1=CC=C(C=C1)CCC(=O)O)C1CC(N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C.CN(C)C(=[N+](C)C)ON1C2=C(C=CC=N2)N=N1.F[P-](F)(F)(F)(F)F.C=1C=CC2=C(C1)N=NN2O.[NH4+].[Cl-].CCN(C(C)C)C(C)C>>C(C)(=O)N(C1=CC=C(C=C1)CCC(=O)N)[C@@H]1C[C@@H](N(C2=...
O[C:27]([CH2:26][CH2:25][c:24]1[cH:23][cH:22][c:21]([N:17]([C@H:16]2[c:15]3[c:10]([cH:11][cH:12][cH:13][cH:14]3)[N:9]([C:7]([c:6]3[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:36][cH:35]3)=[O:8])[C@@H:33]([CH3:34])[CH2:32]2)[C:18]([CH3:19])=[O:20])[cH:31][cH:30]1)=[O:29].[NH4+:28]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([C:7](=[O:8]...
COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(CCC(=O)O)cc3)C[C@@H]2C)cc1.[NH4+]
COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(CCC(N)=O)cc3)C[C@@H]2C)cc1
null
null
CN(C=O)C
Acylation
Carboxylic acid to amide conversion
1283aef55d7ee699f097a8e5267689198c76ba671644401547f902657820236d
cb0a71c3fb37a76e96fbd81aae6f95a28398a03d1ad2c8e877085e735efb98f1
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4].[NH4+;D0:5]>>[C:4]-[C:3]-[C;H0;D3;+0:1](-[NH2;D1;+0:5])=[O;D1;H0:2]
82
[{"value": 82.0, "product": "C(C)(=O)N(C1=CC=C(C=C1)CCC(=O)N)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
(2S,4R)-3-(4-{Acetyl-[1-(4-methoxy-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-amino}-phenyl)-propionamide was prepared from (2S,4R)-3-(4-{Acetyl-[1-(4-methoxy-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-amino}-phenyl)-propionic acid. To a solution of 3-(4-{acetyl-[1-(4-methoxy-benzoyl)-2-methyl-1,2,3,4...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Primary amide
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HO-
CN(C=O)C
null
null
COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(CCC(=O)O)cc3)C[C@@H]2C)cc1.[NH4+]>CN(C=O)C>COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3ccc(CCC(N)=O)cc3)C[C@@H]2C)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0a31dbd4a1ce4c0f8c119144d42ce7ca
COc1cccc(C(=O)N2c3ccccc3C(O)CC2(C)C)c1.Nc1ccccc1>>COc1cccc(C(=O)N2c3ccccc3C(Nc3ccccc3)CC2(C)C)c1
NC1=CC=CC=C1.OC1CC(N(C2=CC=CC=C12)C(=O)C1=CC(=CC=C1)OC)(C)C.I[Si](C)(C)C>>CC1(N(C2=CC=CC=C2C(C1)NC1=CC=CC=C1)C(=O)C1=CC(=CC=C1)OC)C
O[CH:17]1[c:16]2[c:11]([cH:12][cH:13][cH:14][cH:15]2)[N:10]([C:8]([c:7]2[cH:6][cH:5][cH:4][c:3]([O:2][CH3:1])[cH:29]2)=[O:9])[C:26]([CH3:27])([CH3:28])[CH2:25]1.[NH2:18][c:19]1[cH:20][cH:21][cH:22][cH:23][cH:24]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7]([C:8](=[O:9])[N:10]2[c:11]3[cH:12][cH:13][cH:14][cH:15][c:16]3[C...
COc1cccc(C(=O)N2c3ccccc3C(O)CC2(C)C)c1.Nc1ccccc1
COc1cccc(C(=O)N2c3ccccc3C(Nc3ccccc3)CC2(C)C)c1
null
null
ClCCl
Heteroatom Alkylation and Arylation
Reductive amination with alcohol
965275ebca7bef7025897935012fa8cddebfeed57437f060749dfe3d0afc55f2
c4940c2a97a655ce3fe0da51f34327276f5fad64d656fcfdbcd714b6aae5a34d
O=C(c1ccccc1)N1CCC(Nc2ccccc2)c2ccccc21
O-[CH;D3;+0:1]1-[C:2]-[C:3]-[#7:4]-[c:5]:[c:6]-1:[c:7].[NH2;D1;+0:8]-[c:9](:[c:10]):[c:11]>>[c:7]:[c:6]1:[c:5]-[#7:4]-[C:3]-[C:2]-[CH;D3;+0:1]-1-[NH;D2;+0:8]-[c:9](:[c:10]):[c:11]
24.3
[{"value": 24.0, "product": "CC1(N(C2=CC=CC=C2C(C1)NC1=CC=CC=C1)C(=O)C1=CC(=CC=C1)OC)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 24.3, "product": "CC1(N(C2=CC=CC=C2C(C1)NC1=CC=CC=C1)C(=O)C1=CC(=CC=C1)OC)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
6
HOUR
To a chilled solution of (4-hydroxy-2,2-dimethyl-3,4-dihydro-2H-quinolin-1-yl)-(3-methoxy-phenyl)-methanone (500 mg, 1.6 mmol) in 10 ml dichloromethane was added slowly 0.8 ml iodotrimethylsilane (5.6 mmol) at 0° C. The resulting reaction mixture was stirred at 0° C. for 6 hours. Then the mixture was concentrated under...
10.6084/m9.figshare.5104873.v1
null
Secondary alcohol.Primary amine
Secondary amine
c1ccc2c(c1)CCC[NH]2
c1ccc2c(c1)CCC[NH]2
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HO-
ClCCl
0
6
COc1cccc(C(=O)N2c3ccccc3C(O)CC2(C)C)c1.Nc1ccccc1>ClCCl>COc1cccc(C(=O)N2c3ccccc3C(Nc3ccccc3)CC2(C)C)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-742d5628a0184da99e04baf470b05eb8
CC(=O)Cl.COc1cccc(C(=O)N2c3ccccc3C(Nc3ccccc3)CC2(C)C)c1>>COc1cccc(C(=O)N2c3ccccc3C(N(C(C)=O)c3ccccc3)CC2(C)C)c1
O.C(C)(=O)Cl.CC1(N(C2=CC=CC=C2C(C1)NC1=CC=CC=C1)C(=O)C1=CC(=CC=C1)OC)C.C(C)(C)N(CC)C(C)C>>COC=1C=C(C(=O)N2C(CC(C3=CC=CC=C23)N(C(C)=O)C2=CC=CC=C2)(C)C)C=CC1
Cl[C:19]([CH3:20])=[O:21].[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7]([C:8](=[O:9])[N:10]2[c:11]3[cH:12][cH:13][cH:14][cH:15][c:16]3[CH:17]([NH:18][c:22]3[cH:23][cH:24][cH:25][cH:26][cH:27]3)[CH2:28][C:29]2([CH3:30])[CH3:31])[cH:32]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7]([C:8](=[O:9])[N:10]2[c:11]3[cH:12][cH:13][cH:...
CC(=O)Cl.COc1cccc(C(=O)N2c3ccccc3C(Nc3ccccc3)CC2(C)C)c1
COc1cccc(C(=O)N2c3ccccc3C(N(C(C)=O)c3ccccc3)CC2(C)C)c1
null
null
C(Cl)Cl
Acylation
N-alkylation of secondary amines with alkyl halides
b92e0bfd3d683c1f2a209adfe70a67ad7cb0d87749eb59e8fe0cf1689bc291e0
96cb0a2fed10552c5770a45a2d6523b47ac3e38928b4a9c698d8577451182dcd
O=C(c1ccccc1)N1CCC(Nc2ccccc2)c2ccccc21
Cl-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[C:4]-[C:5](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9])-[c:10]>>[C:4]-[C:5](-[N;H0;D3;+0:6](-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3])-[c:7](:[c:8]):[c:9])-[c:10]
null
[]
null
null
null
null
To a solution of (2,2-dimethyl-4-phenylamino-3,4-dihydro-2H-quinolin-1-yl)-(3-methoxy-phenyl)-methanone in methylene chloride (5 mL) was added diisopropylethylamine followed by acetyl chloride. The mixture was stirred at room temperature over night. The mixture was poured into water and extracted with dichloromethane. ...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Secondary amine
Tertiary amide
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HCl
C(Cl)Cl
null
null
CC(=O)Cl.COc1cccc(C(=O)N2c3ccccc3C(Nc3ccccc3)CC2(C)C)c1>C(Cl)Cl>COc1cccc(C(=O)N2c3ccccc3C(N(C(C)=O)c3ccccc3)CC2(C)C)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2d590b77661e4103beba86070db7f71d
CC=O.COc1ccc(C(=O)N2c3ccccc3[C@H](N)C[C@@H]2C)cc1.O=C(Cl)c1ccc(Cl)cc1>>CCN(C(=O)c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(OC)cc2)c2ccccc21
N[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(=O)C1=CC=C(C=C1)OC)C.C(C)=O.C(C)(C)N(C(C)C)CC.ClC1=CC=C(C(=O)Cl)C=C1.C(C)(=O)O[BH-](OC(C)=O)OC(C)=O.[Na+]>>ClC1=CC=C(C(=O)N([C@@H]2C[C@@H](N(C3=CC=CC=C23)C(C2=CC=C(C=C2)OC)=O)C)CC)C=C1
O=[CH:2][CH3:1].[NH2:3][C@@H:13]1[CH2:14][C@H:15]([CH3:16])[N:17]([C:18](=[O:19])[c:20]2[cH:21][cH:22][c:23]([O:24][CH3:25])[cH:26][cH:27]2)[c:28]2[cH:29][cH:30][cH:31][cH:32][c:33]21.Cl[C:4](=[O:5])[c:6]1[cH:7][cH:8][c:9]([Cl:10])[cH:11][cH:12]1>>[CH3:1][CH2:2][N:3]([C:4](=[O:5])[c:6]1[cH:7][cH:8][c:9]([Cl:10])[cH:11]...
CC=O.COc1ccc(C(=O)N2c3ccccc3[C@H](N)C[C@@H]2C)cc1.O=C(Cl)c1ccc(Cl)cc1
CCN(C(=O)c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(OC)cc2)c2ccccc21
null
null
ClCCl
Acylation
OtherReaction
5a782b9f09c0c68997bbc9f3e2598567a6cca607f878381642f196bf4e3a3b46
08f3c3a23435387659fcbdc4547b30dce7a692aa89292d226cb9f3beec91047a
O=C(N[C@@H]1CCN(C(=O)c2ccccc2)c2ccccc21)c1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].O=[CH;D2;+0:6]-[C;D1;H3:7].[C:8]-[C:9](-[NH2;D1;+0:10])-[c:11]>>[C:8]-[C:9](-[N;H0;D3;+0:10](-[CH2;D2;+0:6]-[C;D1;H3:7])-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5])-[c:11]
25.4
[{"value": 24.0, "product": "ClC1=CC=C(C(=O)N([C@@H]2C[C@@H](N(C3=CC=CC=C23)C(C2=CC=C(C=C2)OC)=O)C)CC)C=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 25.4, "product": "ClC1=CC=C(C(=O)N([C@@H]2C[C@@H](N(C3=CC=CC=C23)C(C2=CC=C(C=C2)OC)=O)C)CC)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": fal...
null
null
30
MINUTE
(2S,4R)-4-Chloro-N-ethyl-N-[1-(4-methoxy-benzoyl)-2-methyl-1,2,3,4-tetrahydro-quinolin-4-yl]-benzamide was synthesized as described in general procedure C, except following benzyl carbamate removal the amine was modified in the following manner. To a solution of (2S,4R)-(4-amino-2-methyl-3,4-dihydro-2H-quinolin-1-yl)-(...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Aldehyde.Primary amine
Tertiary amide
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HCl
ClCCl
null
0.5
CC=O.COc1ccc(C(=O)N2c3ccccc3[C@H](N)C[C@@H]2C)cc1.O=C(Cl)c1ccc(Cl)cc1>ClCCl>CCN(C(=O)c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(OC)cc2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5eb6560d5d354efb8accb8043354880f
CC(=O)Cl.COc1ccc(C(=O)N2CCC(Nc3ccccc3)c3ccccc32)cc1>>COc1cccc(C(=O)N2CCC(N(C(C)=O)c3ccccc3)c3ccccc32)c1
O.C(C)(=O)Cl.C1(=CC=CC=C1)NC1CCN(C2=CC=CC=C12)C(=O)C1=CC=C(C=C1)OC.C(C)(C)N(CC)C(C)C>>COC=1C=C(C(=O)N2CCC(C3=CC=CC=C23)N(C(C)=O)C2=CC=CC=C2)C=CC1
Cl[C:15]([CH3:16])=[O:17].[CH3:1][O:2][c:3]1[cH:4][cH:30][c:7]([C:8](=[O:9])[N:10]2[CH2:11][CH2:12][CH:13]([NH:14][c:18]3[cH:19][cH:20][cH:21][cH:22][cH:23]3)[c:24]3[cH:25][cH:26][cH:27][cH:28][c:29]32)[cH:6][cH:5]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7]([C:8](=[O:9])[N:10]2[CH2:11][CH2:12][CH:13]([N:14]([C:15]([CH...
CC(=O)Cl.COc1ccc(C(=O)N2CCC(Nc3ccccc3)c3ccccc32)cc1
COc1cccc(C(=O)N2CCC(N(C(C)=O)c3ccccc3)c3ccccc32)c1
null
null
C(Cl)Cl
Acylation
OtherReaction
5e65d40c7d6c6b6e2f59d40eb17a883d54c27c2d7477ec806a56130f69d6b17e
3db22b1160729ed8a5947d95ae3cc1125e44d4a7f588d068ea1e59774dc755bf
O=C(c1ccccc1)N1CCC(Nc2ccccc2)c2ccccc21
Cl-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[C;D1;H3:4]-[#8:5]-[c;H0;D3;+0:6]1:[cH;D2;+0:7]:[cH;D2;+0:8]:[c:9](-[C:10](=[O;D1;H0:11])-[#7:12]2-[C:13]-[C:14]-[C:15](-[NH;D2;+0:16]-[c:17](:[c:18]):[c:19])-[c:20]:[c:21]-2):[c:22]:[cH;D2;+0:23]:1>>[C;D1;H3:2]-[C;H0;D3;+0:1](=[O;D1;H0:3])-[N;H0;D3;+0:16](-[C:15]1-[C:14]-[C:...
null
[]
null
null
null
null
To a solution of (4-phenylamino-3,4-dihydro-2H-quinolin-1-yl)-(4-methoxy-phenyl)-methanone in methylene chloride was added diisopropylethylamine followed by acetyl chloride. The mixture was stirred at room temperature over night. The mixture was poured into water and extracted with dichloromethane. The extracts were wa...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Ether.Secondary amine
Ether.Tertiary amide
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HCl
C(Cl)Cl
null
null
CC(=O)Cl.COc1ccc(C(=O)N2CCC(Nc3ccccc3)c3ccccc32)cc1>C(Cl)Cl>COc1cccc(C(=O)N2CCC(N(C(C)=O)c3ccccc3)c3ccccc32)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f649d38764ca405192464d9bfecda86b
C[C@@H]1CC(=O)O1.Nc1ccccc1>>C[C@@H](CC(=O)O)Nc1ccccc1
NC1=CC=CC=C1.C1(C[C@@H](C)O1)=O.C(=O)([O-])[O-].[K+].[K+]>>C1(=CC=CC=C1)N[C@H](CC(=O)O)C
[CH3:1][C@@H:2]1[CH2:3][C:4](=[O:5])[O:6]1.[NH2:7][c:8]1[cH:9][cH:10][cH:11][cH:12][cH:13]1>>[CH3:1][C@@H:2]([CH2:3][C:4](=[O:5])[OH:6])[NH:7][c:8]1[cH:9][cH:10][cH:11][cH:12][cH:13]1
C[C@@H]1CC(=O)O1.Nc1ccccc1
C[C@@H](CC(=O)O)Nc1ccccc1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
0ecd4f20532980ca9a1e759f7de022b3f8b73a123ab3bb9fa09d76ccf580e32d
73c1447270f630809b051744bf93d0489db5238d09a5e3d5f3ef6001adc8b63b
c1ccccc1
[C;D1;H3:1]-[C@@H;D3;+0:2]1-[C:3]-[C:4](=[O;D1;H0:5])-[O;H0;D2;+0:6]-1.[NH2;D1;+0:7]-[c:8](:[c:9]):[c:10]>>[C;D1;H3:1]-[C@@H;D3;+0:2](-[C:3]-[C:4](=[O;D1;H0:5])-[OH;D1;+0:6])-[NH;D2;+0:7]-[c:8](:[c:9]):[c:10]
null
[]
80.85
CELSIUS
null
null
A jacketed 30-L 3-neck bottom-valve cylindrical reactor equipped with overhead stirrer, reflux condenser, addition funnel, and N2 inlet was flushed with N2. Water (8.7 L) was charged followed by aniline (423 L, 4.9 mol). Stirring was initiated and the internal temperature set for 80° C. After the internal temperature r...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine
Carboxylic acid.Secondary amine
C1COC1
null
c1ccccc1
null
null
80.85
null
C[C@@H]1CC(=O)O1.Nc1ccccc1>>C[C@@H](CC(=O)O)Nc1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5ac1040694054d8ca141260d7b6e629a
CCOC(C)=O.C[C@H]1C[C@@H](N)c2ccccc2N1C(=O)c1ccc(F)cc1.OB(O)c1ccc(Cl)cc1>>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccccc21
C(C)(=O)OCC.N[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(=O)C1=CC=C(C=C1)F)C.ClC1=CC=C(C=C1)B(O)O.N1=CC=CC=C1>>ClC1=CC=C(C=C1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)F)=O)C
CCO[C:2]([CH3:1])=[O:3].[NH2:4][C@@H:12]1[CH2:13][C@H:14]([CH3:15])[N:16]([C:17](=[O:18])[c:19]2[cH:20][cH:21][c:22]([F:23])[cH:24][cH:25]2)[c:26]2[cH:27][cH:28][cH:29][cH:30][c:31]21.OB(O)[c:5]1[cH:6][cH:7][c:8]([Cl:9])[cH:10][cH:11]1>>[CH3:1][C:2](=[O:3])[N:4]([c:5]1[cH:6][cH:7][c:8]([Cl:9])[cH:10][cH:11]1)[C@@H:12]1...
CCOC(C)=O.C[C@H]1C[C@@H](N)c2ccccc2N1C(=O)c1ccc(F)cc1.OB(O)c1ccc(Cl)cc1
CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccccc21
null
C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-]
CN(C)C=O
Acylation
OtherReaction
d5b79df0bcad37b68666465f98bdbf09561dfcc3b18a2acc5b3be323501cddff
d21a41b88b3a6857658a80208e904dc455b890b23aaf7d742d8a593a93afbd98
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
C-C-O-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].O-B(-O)-[c;H0;D3;+0:4](:[c:5]:[c:6]):[c:7]:[c:8].[C:9]-[C:10](-[NH2;D1;+0:11])-[c:12]>>[C:9]-[C:10](-[N;H0;D3;+0:11](-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3])-[c;H0;D3;+0:4](:[c:5]:[c:6]):[c:7]:[c:8])-[c:12]
18
[{"value": 18.0, "product": "ClC1=CC=C(C=C1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)F)=O)C", "details": "PERCENTYIELD", "is_desired": false}]
60
CELSIUS
1
HOUR
To a solution of (2S,4R)-(4-amino-2-methyl-3,4-dihydro-2H-quinolin-1-yl)-(4-fluoro-phenyl)-methanone (1.0 g, 3.5 mmol) in DMF (20 mL, dry) was added 4-chlorophenylboronic acid (1.1 g, 7.0 mmol), pyridine (850 uL, 10.5 mmol) and copper(II)acetate (1.27 g, 7.0 mmol). The heterogeneous green mixture was stirred open to ai...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine.Boronic acid
Tertiary amide
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HO-.B
C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-].CN(C)C=O
60
1
CCOC(C)=O.C[C@H]1C[C@@H](N)c2ccccc2N1C(=O)c1ccc(F)cc1.OB(O)c1ccc(Cl)cc1>C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-].CN(C)C=O>CC(=O)N(c1ccc(Cl)cc1)[C@@H]1C[C@H](C)N(C(=O)c2ccc(F)cc2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7d5cd33344af40e2a4eb5b7e6e8f6f65
CC(=O)Cl.C[C@H]1C[C@@H](Nc2ccc(Cl)cc2)c2ccccc2N1C(=O)c1ccc(F)cc1>>CC(=O)N(c1ccc(Cl)cc1)C1CC(C)N(C(=O)c2ccc(F)cc2)c2ccccc21
ClC1=CC=C(C=C1)N[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(=O)C1=CC=C(C=C1)F)C.C(C)(C)N(CC)C(C)C.C(C)(=O)Cl>>ClC1=CC=C(C=C1)N(C(C)=O)C1CC(N(C2=CC=CC=C12)C(C1=CC=C(C=C1)F)=O)C
Cl[C:2]([CH3:1])=[O:3].[NH:4]([c:5]1[cH:6][cH:7][c:8]([Cl:9])[cH:10][cH:11]1)[C@@H:12]1[CH2:13][C@H:14]([CH3:15])[N:16]([C:17](=[O:18])[c:19]2[cH:20][cH:21][c:22]([F:23])[cH:24][cH:25]2)[c:26]2[cH:27][cH:28][cH:29][cH:30][c:31]21>>[CH3:1][C:2](=[O:3])[N:4]([c:5]1[cH:6][cH:7][c:8]([Cl:9])[cH:10][cH:11]1)[CH:12]1[CH2:13]...
CC(=O)Cl.C[C@H]1C[C@@H](Nc2ccc(Cl)cc2)c2ccccc2N1C(=O)c1ccc(F)cc1
CC(=O)N(c1ccc(Cl)cc1)C1CC(C)N(C(=O)c2ccc(F)cc2)c2ccccc21
null
null
null
Acylation
N-alkylation of secondary amines with alkyl halides
b92e0bfd3d683c1f2a209adfe70a67ad7cb0d87749eb59e8fe0cf1689bc291e0
96cb0a2fed10552c5770a45a2d6523b47ac3e38928b4a9c698d8577451182dcd
O=C(c1ccccc1)N1CCC(Nc2ccccc2)c2ccccc21
Cl-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[c:4]:[c:5](-[NH;D2;+0:6]-[C@@H;D3;+0:7]1-[C:8]-[C:9]-[#7:10]-[c:11]:[c:12]-1:[c:13]):[c:14]>>[C;D1;H3:2]-[C;H0;D3;+0:1](=[O;D1;H0:3])-[N;H0;D3;+0:6](-[CH;D3;+0:7]1-[C:8]-[C:9]-[#7:10]-[c:11]:[c:12]-1:[c:13])-[c:5](:[c:4]):[c:14]
71
[{"value": 71.0, "product": "ClC1=CC=C(C=C1)N(C(C)=O)C1CC(N(C2=CC=CC=C12)C(C1=CC=C(C=C1)F)=O)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
To a solution of (2S,4R)-[4-(4-chloro-phenylamino)-2-methyl-3,4-dihydro-2H-quinolin-1-yl]-(4-fluoro-phenyl)-methanone (250 mg, 0.636 mmol) in acetyl chloride (5 mL) was added diisopropylethylamine (120 uL, 0.70 mmol). The mixture was stirred at rt 4 h. The mixture was concentrated under reduced pressure, dissolved in e...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Secondary amine
Tertiary amide
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HCl
null
null
4
CC(=O)Cl.C[C@H]1C[C@@H](Nc2ccc(Cl)cc2)c2ccccc2N1C(=O)c1ccc(F)cc1>>CC(=O)N(c1ccc(Cl)cc1)C1CC(C)N(C(=O)c2ccc(F)cc2)c2ccccc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9b1f9a27aafd474ebbeca7ef6221b5ab
COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3cccc(C#N)c3)C[C@@H]2C)cc1>>COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3cccc(CN)c3)C[C@@H]2C)cc1
C(#N)C=1C=C(C=CC1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C.[BH4-].[Na+]>>NCC=1C=C(C=CC1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C
[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([C:7](=[O:8])[N:9]2[c:10]3[cH:11][cH:12][cH:13][cH:14][c:15]3[C@H:16]([N:17]([C:18]([CH3:19])=[O:20])[c:21]3[cH:22][cH:23][cH:24][c:25]([C:26]#[N:27])[cH:28]3)[CH2:29][C@@H:30]2[CH3:31])[cH:32][cH:33]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([C:7](=[O:8])[N:9]2[c:10]3[cH:11][cH:12][cH:1...
COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3cccc(C#N)c3)C[C@@H]2C)cc1
COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3cccc(CN)c3)C[C@@H]2C)cc1
null
[Co](Cl)Cl
null
Reduction
Reduction of nitrile to amine
65bec2d9f430701d30dc9fcbe1c5418f3dfa174d67be035c50edfc71895dc9c7
e8d1bc928b94bd4f5bf4b23363ce8f88b1ce7d146ba93829e7b8ad8dbe0007a7
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
[N;H0;D1;+0:1]#[C;H0;D2;+0:2]-[c:3](:[c:4]):[c:5]>>[NH2;D1;+0:1]-[CH2;D2;+0:2]-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
N-(3-cyanophenyl)-N-[(2S,4R)-1-(4-methoxybenzoyl)-2-methyl-1,2,3,4-tetrahydroquinolin-4-yl]acetamide was further treated with cobalt(II)chloride and sodium borohydride (1 eq, 3 eq) to afford N-[3-(aminomethyl)phenyl]-N-[(2S,4R)-1-(4-methoxybenzoyl)-2-methyl-1,2,3,4-tetrahydroquinolin-4-yl]acetamide. Conditions: See rea...
10.6084/m9.figshare.5104873.v1
null
Nitrile
Primary amine
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
null
[Co](Cl)Cl
null
null
COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3cccc(C#N)c3)C[C@@H]2C)cc1>[Co](Cl)Cl>COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3cccc(CN)c3)C[C@@H]2C)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-90dfa87f2f53498d924aed3d71d1ebad
COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3cccc(CN)c3)C[C@@H]2C)cc1.O=C(O)CO>>COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3cccc(CNC(=O)CO)c3)C[C@@H]2C)cc1
C=1C=CC2=C(C1)N=NN2O.NCC=1C=C(C=CC1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C.C(CO)(=O)O.CCN=C=NCCCN(C)C>>C(CO)(=O)NCC=1C=C(C=CC1)N(C(C)=O)[C@@H]1C[C@@H](N(C2=CC=CC=C12)C(C1=CC=C(C=C1)OC)=O)C
[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([C:7](=[O:8])[N:9]2[c:10]3[cH:11][cH:12][cH:13][cH:14][c:15]3[C@H:16]([N:17]([C:18]([CH3:19])=[O:20])[c:21]3[cH:22][cH:23][cH:24][c:25]([CH2:26][NH2:27])[cH:32]3)[CH2:33][C@@H:34]2[CH3:35])[cH:36][cH:37]1.O=[C:28]([OH:29])[CH2:30][OH:31]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([C:7](=[O...
COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3cccc(CN)c3)C[C@@H]2C)cc1.O=C(O)CO
COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3cccc(CNC(=O)CO)c3)C[C@@H]2C)cc1
null
null
null
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(c1ccccc1)N1CC[C@@H](Nc2ccccc2)c2ccccc21
O=[C;H0;D3;+0:1](-[OH;D1;+0:2])-[C:3]-[O;D1;H1:4].[NH2;D1;+0:5]-[C:6]-[c:7]>>[O;D1;H1:4]-[C:3]-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[NH;D2;+0:5]-[C:6]-[c:7]
null
[]
null
null
null
null
N-[3-(aminomethyl)phenyl]-N-[(2S,4R)-1-(4-methoxybenzoyl)-2-methyl-1,2,3,4-tetrahydroquinolin-4-yl]acetamide was then further coupled with glycolic acid using coupling reagent such as EDCI with HOBt to afford N-{3-[(glycoloylamino)methyl]phenyl}-N-[(2S,4R)-1-(4-methoxybenzoyl)-2-methyl-1,2,3,4-tetrahydroquinolin-4-yl]a...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccccc1.c1ccc2c(c1)CCC[NH]2
HO-
null
null
null
COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3cccc(CN)c3)C[C@@H]2C)cc1.O=C(O)CO>>COc1ccc(C(=O)N2c3ccccc3[C@H](N(C(C)=O)c3cccc(CNC(=O)CO)c3)C[C@@H]2C)cc1