dataset_id
large_stringclasses
414 values
reaction_id
large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
reactant_smiles
large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-067378496b04452e821815e4bd116d99
CCCCCn1c(=S)[nH]c(=O)c2[nH]c(C(F)(F)F)nc21.COS(=O)(=O)OC>>CCCCCn1c(SC)nc(=O)c2[nH]c(C(F)(F)F)nc21
C(CCCC)N1C(NC(C=2NC(=NC12)C(F)(F)F)=O)=S.[OH-].[Na+].S(=O)(=O)(OC)OC>>CSC1=NC(C=2NC(=NC2N1CCCCC)C(F)(F)F)=O
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7](=[S:8])[nH:10][c:11](=[O:12])[c:13]2[nH:14][c:15]([C:16]([F:17])([F:18])[F:19])[n:20][c:21]12.COS(=O)(=O)O[CH3:9]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]([S:8][CH3:9])[n:10][c:11](=[O:12])[c:13]2[nH:14][c:15]([C:16]([F:17])([F:18])[F:19])[n:20][c:21]12
CCCCCn1c(=S)[nH]c(=O)c2[nH]c(C(F)(F)F)nc21.COS(=O)(=O)OC
CCCCCn1c(SC)nc(=O)c2[nH]c(C(F)(F)F)nc21
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
0161fed9f1388ec369b7cbafe281cc52a2e7ee362447238b9354e3768807eefa
e73b6e23c9de2770653dfe1c031448ae08eae1a1e8b31e289bfc4b4719e52064
O=c1nc[nH]c2nc[nH]c12
C-O-S(=O)(=O)-O-[CH3;D1;+0:1].[C:2]-[#7;a:3]1:[c:4]2:[#7;a:5]:[c:6]:[#7;a:7]:[c:8]:2:[c:9](=[O;D1;H0:10]):[nH;D2;+0:11]:[c;H0;D3;+0:12]:1=[S;H0;D1;+0:13]>>[C:2]-[#7;a:3]1:[c:4]2:[#7;a:5]:[c:6]:[#7;a:7]:[c:8]:2:[c:9](=[O;D1;H0:10]):[n;H0;D2;+0:11]:[c;H0;D3;+0:12]:1-[S;H0;D2;+0:13]-[CH3;D1;+0:1]
95.6
[{"value": 95.6, "product": "CSC1=NC(C=2NC(=NC2N1CCCCC)C(F)(F)F)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 93.7, "product": "CSC1=NC(C=2NC(=NC2N1CCCCC)C(F)(F)F)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1.5
HOUR
To the solution of 3-pentyl-2-thioxo-8-(trifluoromethyl)-1,2,3,7-tetrahydro-6H-purin-6-one (600 mg, 2 mmol) in a 2 M solution of sodium hydroxide in water (12.0 mL) was added dimethyl sulfate (0.30 mL, 3.2 mmol). The reaction mixture was stirred at room temperature for 1.5 h and quenched with acetic acid. The resulting...
10.6084/m9.figshare.5104873.v1
null
Thiocarbonyl
Monosulfide
c1ncc2[nH]cnc2n1
c1ncc2[nH]cnc2n1
c1ncc2[nH]cnc2n1
HO-
O
null
1.5
CCCCCn1c(=S)[nH]c(=O)c2[nH]c(C(F)(F)F)nc21.COS(=O)(=O)OC>O>CCCCCn1c(SC)nc(=O)c2[nH]c(C(F)(F)F)nc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-838894972a19416c8dc5bca23021abb4
CCCCCN1c2nc(C(F)(F)F)[nH]c2C(=O)NC1SC.NN>>CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]c(C(F)(F)F)nc21
CSC1NC(C=2NC(=NC2N1CCCCC)C(F)(F)F)=O.NN>>C(CCCC)N1/C(/NC(C=2NC(=NC12)C(F)(F)F)=O)=N/N
CS[CH:7]1[N:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:21]2[c:13]([nH:14][c:15]([C:16]([F:17])([F:18])[F:19])[n:20]2)[C:11](=[O:12])[NH:10]1.[NH2:8][NH2:9]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1/[c:7](=[N:8]/[NH2:9])[nH:10][c:11](=[O:12])[c:13]2[nH:14][c:15]([C:16]([F:17])([F:18])[F:19])[n:20][c:21]12
CCCCCN1c2nc(C(F)(F)F)[nH]c2C(=O)NC1SC.NN
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]c(C(F)(F)F)nc21
null
null
O
Miscellaneous
OtherReaction
95e6ec4ef33bb106a3bdb58795cc57ba37baa15165453addc14097b6a24c5025
2ba1ac28c36a0747dfaa43d922f0b0fd42ee3ff9c9f7e15186668fec5629e33f
N=c1[nH]c(=O)c2[nH]cnc2[nH]1
C-S-[CH;D3;+0:1]1-[NH;D2;+0:2]-[C;H0;D3;+0:3](=[O;D1;H0:4])-[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2-[N;H0;D3;+0:10]-1-[C:11]-[C:12].[N;D1;H2:13]-[NH2;D1;+0:14]>>[C:12]-[C:11]-[n;H0;D3;+0:10]1:[c:9]2:[#7;a:8]:[c:7]:[#7;a:6]:[c:5]:2:[c;H0;D3;+0:3](=[O;D1;H0:4]):[nH;D2;+0:2]/[c;H0;D3;+0:1]:1=[N;H0;D2;+0:14]\[N;D1;H2:13]
86.5
[{"value": 65.0, "product": "C(CCCC)N1/C(/NC(C=2NC(=NC12)C(F)(F)F)=O)=N/N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 86.5, "product": "C(CCCC)N1/C(/NC(C=2NC(=NC12)C(F)(F)F)=O)=N/N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
1
HOUR
A mixture of 2-(methylthio)-3-pentyl-8-(trifluoromethyl)-1,2,3,7-tetrahydro-6H-purin-6-one (0.61 g, 0.95 mmol), hydrazine (3 mL, 100 mmol) and water (3 mL) was stirred at 100° C. for 1 h. The reaction solution was concentrated under reduced pressure. The residue was dissolved in DMSO and purified by preparative LCMS. T...
10.6084/m9.figshare.5104873.v1
null
Hydrazine.Secondary amide.Tertiary amine.Monosulfide
Hydrazone
c1nc2c(n1)[N]CNC2
c1ncc2[nH]cnc2n1
c1ncc2[nH]cnc2n1
Other
O
100
1
CCCCCN1c2nc(C(F)(F)F)[nH]c2C(=O)NC1SC.NN>O>CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]c(C(F)(F)F)nc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7460d3dbb3654fe8ac42ae7a7e072513
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]c(C(F)(F)F)nc21.CCOC(C)(OCC)OCC>>CCCCCn1c2nc(C(F)(F)F)[nH]c2c(=O)n2c(C)nnc12
C(CCCC)N1/C(/NC(C=2NC(=NC12)C(F)(F)F)=O)=N/N.C(C)(OCC)(OCC)OCC>>CC1=NN=C2N1C(C=1NC(=NC1N2CCCCC)C(F)(F)F)=O
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([C:10]([F:11])([F:12])[F:13])[nH:14][c:15]2[c:16](=[O:17])[nH:18]/[c:23]1=[N:22]\[NH2:21].CCO[C:19](OCC)(OCC)[CH3:20]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([C:10]([F:11])([F:12])[F:13])[nH:14][c:15]2[c:16](=[O:17])[n:18]2[c:19]([CH3:20])[n:2...
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]c(C(F)(F)F)nc21.CCOC(C)(OCC)OCC
CCCCCn1c2nc(C(F)(F)F)[nH]c2c(=O)n2c(C)nnc12
null
null
null
Aromatic Heterocycle Formation
OtherReaction
ee0085044cada96f0b435a4156edc12d66c02309699c14d468ea3b7289b478ad
d53861995bb64d247d09c3f779c372454b394f82c16bc2582c721d04267c3478
O=c1c2[nH]cnc2[nH]c2nncn12
C-C-O-[C;H0;D4;+0:1](-[C;D1;H3:2])(-O-C-C)-O-C-C.[C:3]-[#7;a:4]1:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:[c:10](=[O;D1;H0:11]):[nH;D2;+0:12]/[c;H0;D3;+0:13]:1=[N;H0;D2;+0:14]\[NH2;D1;+0:15]>>[C:3]-[#7;a:4]1:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:[c:10](=[O;D1;H0:11]):[n;H0;D3;+0:12]2:[c;H0;D3;+0:1](-[C;D1;H3:2]):[n;H0;D...
null
[]
null
null
1
HOUR
A mixture of (2E)-3-pentyl-8-(trifluoromethyl)-3,7-dihydro-1H-purine-2,6-dione-2-hydrazone (0.020 g, 0.14 mmol) and triethyl orthoacetate (2 mL, 10 mmol) was stirred at room temperature for 1 h. The reaction mixture was concentrated under vacuum and the residue was purified by preparative LCMS. The product fractions we...
10.6084/m9.figshare.5104873.v1
null
Hydrazone.Ether.Ether.Ether
null
c1ncc2nc[nH]c2n1
c1nc2cn3cnnc3nc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
HO-
null
null
1
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]c(C(F)(F)F)nc21.CCOC(C)(OCC)OCC>>CCCCCn1c2nc(C(F)(F)F)[nH]c2c(=O)n2c(C)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7bf8b5b452ce4684a8db2a4c4c018f0c
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]c(C(F)(F)F)nc21>>CCCCCn1c2nc(C(F)(F)F)[nH]c2c(=O)n2cnnc12
C(CCCC)N1/C(/NC(C=2NC(=NC12)C(F)(F)F)=O)=N/N.C(OCC)(OCC)OCC>>C(CCCC)N1C=2N(C(C=3NC(=NC13)C(F)(F)F)=O)C=NN2
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([C:10]([F:11])([F:12])[F:13])[nH:14][c:15]2[c:16](=[O:17])[nH:18]/[c:22]1=[N:21]\[NH2:20]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([C:10]([F:11])([F:12])[F:13])[nH:14][c:15]2[c:16](=[O:17])[n:18]2[cH:19][n:20][n:21][c:22]12
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]c(C(F)(F)F)nc21
CCCCCn1c2nc(C(F)(F)F)[nH]c2c(=O)n2cnnc12
null
null
null
Aromatic Heterocycle Formation
OtherReaction
60a3d12ea17afaadb59a56b0f52041f740243ef406a6802686b793ec22e80d0f
d627647f8a5758e4c676083258d3a8813f47848ab7ceb334945a07e482fcef85
O=c1c2[nH]cnc2[nH]c2nncn12
[C:1]-[#7;a:2]1:[c:3]2:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:2:[c:8](=[O;D1;H0:9]):[nH;D2;+0:10]/[c;H0;D3;+0:11]:1=[N;H0;D2;+0:12]\[NH2;D1;+0:13]>>[C:1]-[#7;a:2]1:[c:3]2:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:2:[c:8](=[O;D1;H0:9]):[n;H0;D3;+0:10]2:[c:14]:[n;H0;D2;+0:13]:[n;H0;D2;+0:12]:[c;H0;D3;+0:11]:1:2
227.3
[{"value": 48.0, "product": "C(CCCC)N1C=2N(C(C=3NC(=NC13)C(F)(F)F)=O)C=NN2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 227.3, "product": "C(CCCC)N1C=2N(C(C=3NC(=NC13)C(F)(F)F)=O)C=NN2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
A mixture of (2E)-3-pentyl-8-(trifluoromethyl)-3,7-dihydro-1H-purine-2,6-dione-2-hydrazone (0.020 g, 0.14 mmol) and triethyl orthoformate (2 mL, 0.01 mol) was stirred at room temperature for 1 h. The reaction mixture was concentrated under vacuum and the residue was purified by preparative LCMS. The product fractions w...
10.6084/m9.figshare.5104873.v1
null
Hydrazone
null
c1ncc2nc[nH]c2n1
c1nc2cn3cnnc3nc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
Other
null
null
1
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]c(C(F)(F)F)nc21>>CCCCCn1c2nc(C(F)(F)F)[nH]c2c(=O)n2cnnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-30172eddcbc441a6ac8a88d2eff42fac
CCCCC=O.NC(=O)c1[nH]cnc1N>>CCCCCNc1nc[nH]c1C(N)=O
NC=1N=CNC1C(=O)N.C(CCCC)=O.C(#N)[BH3-].[Na+]>>C(CCCC)NC=1N=CNC1C(=O)N
O=[CH:5][CH2:4][CH2:3][CH2:2][CH3:1].[NH2:6][c:7]1[n:8][cH:9][nH:10][c:11]1[C:12]([NH2:13])=[O:14]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][NH:6][c:7]1[n:8][cH:9][nH:10][c:11]1[C:12]([NH2:13])=[O:14]
CCCCC=O.NC(=O)c1[nH]cnc1N
CCCCCNc1nc[nH]c1C(N)=O
null
null
CO
Heteroatom Alkylation and Arylation
Reductive amination with aldehyde
422be648aea52bce28ccc8fb32ec3178aaa47bbd624f063874619362f075b5f2
7915721a3e395aed85e3c40dc4d725c571a931ac517c6a0da16f2a2b0bb5eac7
c1c[nH]cn1
O=[CH;D2;+0:1]-[C:2]-[C:3].[N;D1;H2:4]-[C:5](=[O;D1;H0:6])-[c:7]1:[#7;a:8]:[c:9]:[#7;a:10]:[c:11]:1-[NH2;D1;+0:12]>>[C:3]-[C:2]-[CH2;D2;+0:1]-[NH;D2;+0:12]-[c:11]1:[#7;a:10]:[c:9]:[#7;a:8]:[c:7]:1-[C:5](-[N;D1;H2:4])=[O;D1;H0:6]
65.7
[{"value": 63.1, "product": "C(CCCC)NC=1N=CNC1C(=O)N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 65.7, "product": "C(CCCC)NC=1N=CNC1C(=O)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
4-Amino-1H-imidazole-5-carboxamide (13.0 g, 0.104 mol) and valeraldehyde (11 mL, 0.10 mol) were mixed in methanol (200 mL). After being stirred for 30 min, sodium cyanoborohydride (6.5 g, 0.10 mol) was added to the solution and stirring was continued overnight. The reaction mixture was concentrated under reduced pressu...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary amine
Secondary amine
null
null
c1c[nH]cn1
Other
CO
null
0.5
CCCCC=O.NC(=O)c1[nH]cnc1N>CO>CCCCCNc1nc[nH]c1C(N)=O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6998397603674178bb5187b16f13eace
CCCCCNc1nc[nH]c1C(N)=O.O=C(N=C=S)c1ccccc1>>CCCCCN(C(=S)NC(=O)c1ccccc1)c1nc[nH]c1C(N)=O
C(CCCC)NC=1N=CNC1C(=O)N.C(C1=CC=CC=C1)(=O)N=C=S>>C(C1=CC=CC=C1)(=O)NC(=S)N(C=1N=CNC1C(=O)N)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][NH:6][c:18]1[n:19][cH:20][nH:21][c:22]1[C:23]([NH2:24])=[O:25].[C:7](=[S:8])=[N:9][C:10](=[O:11])[c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][N:6]([C:7](=[S:8])[NH:9][C:10](=[O:11])[c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1)[c:18]1[n:19][cH:20][nH...
CCCCCNc1nc[nH]c1C(N)=O.O=C(N=C=S)c1ccccc1
CCCCCN(C(=S)NC(=O)c1ccccc1)c1nc[nH]c1C(N)=O
null
null
C(Cl)Cl
Heteroatom Alkylation and Arylation
thiourea
16b9dd18807f693b1cdd004c800af858aba15692e46e0e83fca1718f8bcadabb
48e0e6261e922bdea79c78ea511461d733cbd49c10100c782d86c83675c4be7c
O=C(NC(=S)Nc1c[nH]cn1)c1ccccc1
[C:1]-[C:2]-[NH;D2;+0:3]-[c:4]1:[#7;a:5]:[c:6]:[#7;a:7]:[c:8]:1-[C:9](-[N;D1;H2:10])=[O;D1;H0:11].[O;D1;H0:12]=[C:13](-[c:14])-[N;H0;D2;+0:15]=[C;H0;D2;+0:16]=[S;D1;H0:17]>>[C:1]-[C:2]-[N;H0;D3;+0:3](-[C;H0;D3;+0:16](=[S;D1;H0:17])-[NH;D2;+0:15]-[C:13](=[O;D1;H0:12])-[c:14])-[c:4]1:[#7;a:5]:[c:6]:[#7;a:7]:[c:8]:1-[C:9]...
139.1
[{"value": 80.0, "product": "C(C1=CC=CC=C1)(=O)NC(=S)N(C=1N=CNC1C(=O)N)CCCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 139.1, "product": "C(C1=CC=CC=C1)(=O)NC(=S)N(C=1N=CNC1C(=O)N)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To a solution of 4-(pentylamino)-1H-imidazole-5-carboxamide (4.0 g, 0.020 mol) in DCM (50 mL) was added benzoyl isothiocyanate (3.3 mL, 0.024 mol). After being stirred overnight, the solid formed was filtered to give the crude product (10 g, ca 60% purity, 80% yield). This product was used for next step without further...
10.6084/m9.figshare.5104873.v1
null
Secondary amine.Isothiocyanate
Thiourea
null
null
c1ccccc1.c1c[nH]cn1
null
C(Cl)Cl
null
8
CCCCCNc1nc[nH]c1C(N)=O.O=C(N=C=S)c1ccccc1>C(Cl)Cl>CCCCCN(C(=S)NC(=O)c1ccccc1)c1nc[nH]c1C(N)=O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c4e9d8453a0f47fab13d4cea37fbad55
CCCCCN(C(=S)NC(=O)c1ccccc1)c1nc[nH]c1C(N)=O>>CCCCCn1c(=S)[nH]c(=O)c2[nH]cnc21
C(C1=CC=CC=C1)(=O)NC(=S)N(C=1N=CNC1C(=O)N)CCCCC.[OH-].[Na+].Cl>>C(CCCC)N1C(NC(C=2NC=NC12)=O)=S
O=C(N[C:7]([N:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:16]1[c:12]([C:10]([NH2:9])=[O:11])[nH:13][cH:14][n:15]1)=[S:8])c1ccccc1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7](=[S:8])[nH:9][c:10](=[O:11])[c:12]2[nH:13][cH:14][n:15][c:16]12
CCCCCN(C(=S)NC(=O)c1ccccc1)c1nc[nH]c1C(N)=O
CCCCCn1c(=S)[nH]c(=O)c2[nH]cnc21
null
null
O
Miscellaneous
OtherReaction
0252aefeec8e267f50de46810e919c261b4cb308e945d000117b9bcb9d1582e0
9e0b04c616da96e0a2af4ca4b9d4b3bbdfbb764c8e3965d78a6a9136f6c866ee
O=c1[nH]c(=S)[nH]c2nc[nH]c12
O=C(-N-[C;H0;D3;+0:1](=[S;D1;H0:2])-[N;H0;D3;+0:3](-[C:4]-[C:5])-[c:6]1:[#7;a:7]:[c:8]:[#7;a:9]:[c:10]:1-[C;H0;D3;+0:11](-[NH2;D1;+0:12])=[O;D1;H0:13])-c1:c:c:c:c:c:1>>[C:5]-[C:4]-[n;H0;D3;+0:3]1:[c:6]2:[#7;a:7]:[c:8]:[#7;a:9]:[c:10]:2:[c;H0;D3;+0:11](=[O;D1;H0:13]):[nH;D2;+0:12]:[c;H0;D3;+0:1]:1=[S;D1;H0:2]
94
[{"value": 94.0, "product": "C(CCCC)N1C(NC(C=2NC=NC12)=O)=S", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 4-[[(benzoylamino)carbonothioyl](pentyl)amino]-1H-imidazole-5-carboxamide (11.8 g, 0.0263 mol) and 1 M of sodium hydroxide in water (75 mL) was heated to reflux for 3 h. Solid was formed in the reaction mixture. The reaction mixture was adjusted to pH 3-4 with concentrated HCl with cooling in an ice bath. ...
10.6084/m9.figshare.5104873.v1
null
Thiourea.Primary amide.Secondary amide
Thiocarbonyl
c1c[nH]cn1.c1ccccc1
c1ncc2[nH]cnc2n1
c1ncc2[nH]cnc2n1
HO-
O
null
null
CCCCCN(C(=S)NC(=O)c1ccccc1)c1nc[nH]c1C(N)=O>O>CCCCCn1c(=S)[nH]c(=O)c2[nH]cnc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-c5affaf43c70471d821746c1e957c5ee
CCCCCn1c(=S)[nH]c(=O)c2[nH]cnc21.NN>>CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21
C(CCCC)N1C(NC(C=2NC=NC12)=O)=S.NN>>C(CCCC)N1/C(/NC(C=2NC=NC12)=O)=N/N
S=[c:7]1[n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:17]2[c:13]([c:11](=[O:12])[nH:10]1)[nH:14][cH:15][n:16]2.[NH2:8][NH2:9]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1/[c:7](=[N:8]/[NH2:9])[nH:10][c:11](=[O:12])[c:13]2[nH:14][cH:15][n:16][c:17]12
CCCCCn1c(=S)[nH]c(=O)c2[nH]cnc21.NN
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
2e80fee15f068129596c03f86e4a84f3567a03df4d28de9eb824e4b8de606d19
b31709867bbae7bd190a95c324309111afc274c1ce2b8bd283fc7d83feae5185
N=c1[nH]c(=O)c2[nH]cnc2[nH]1
S=[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4](:[#7;a:5]):[c:6](:[#7;a:7]):[#7;a:8]:1-[C:9].[N;D1;H2:10]-[NH2;D1;+0:11]>>[#7;a:5]:[c:4]1:[c:3]:[#7;a:2]/[c;H0;D3;+0:1](=[N;H0;D2;+0:11]\[N;D1;H2:10]):[#7;a:8](-[C:9]):[c:6]:1:[#7;a:7]
79.4
[{"value": 78.0, "product": "C(CCCC)N1/C(/NC(C=2NC=NC12)=O)=N/N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 79.4, "product": "C(CCCC)N1/C(/NC(C=2NC=NC12)=O)=N/N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
null
null
3-Pentyl-2-thioxo-1,2,3,7-tetrahydro-6H-purin-6-one (6.0 g, 16 mmol) was mixed with hydrazine (10 mL, 300 mmol) and water (10 mL). The mixture was heated at 100° C. for 8 h. The solid formed was filtered and washed with water to give the desired product (3.0 g, 78%). LCMS calculated for C10H17N6O (M+H): 237.1; found: 2...
10.6084/m9.figshare.5104873.v1
null
Hydrazine.Thiocarbonyl
Hydrazone
c1ncc2[nH]cnc2n1
c1ncc2[nH]cnc2n1
c1ncc2[nH]cnc2n1
Other
O
100
null
CCCCCn1c(=S)[nH]c(=O)c2[nH]cnc21.NN>O>CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b8a05952f69a45aab60bfdaad89b588e
CCCCCn1/c(=N\N)[nH]c(=O)c2[nH]cnc21.CCOC(C)(OCC)OCC>>CCCCCn1c2nc[nH]c2c(=O)n2c(C)nnc12
C(CCCC)N1\C(\NC(C=2NC=NC12)=O)=N/N.C(C)(OCC)(OCC)OCC>>CC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[nH:14]/[c:19]1=[N:18]/[NH2:17].CCO[C:15](OCC)(OCC)[CH3:16]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[n:14]2[c:15]([CH3:16])[n:17][n:18][c:19]12
CCCCCn1/c(=N\N)[nH]c(=O)c2[nH]cnc21.CCOC(C)(OCC)OCC
CCCCCn1c2nc[nH]c2c(=O)n2c(C)nnc12
null
null
null
Aromatic Heterocycle Formation
OtherReaction
ee0085044cada96f0b435a4156edc12d66c02309699c14d468ea3b7289b478ad
d53861995bb64d247d09c3f779c372454b394f82c16bc2582c721d04267c3478
O=c1c2[nH]cnc2[nH]c2nncn12
C-C-O-[C;H0;D4;+0:1](-[C;D1;H3:2])(-O-C-C)-O-C-C.[C:3]-[#7;a:4]1:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:[c:10](=[O;D1;H0:11]):[nH;D2;+0:12]/[c;H0;D3;+0:13]:1=[N;H0;D2;+0:14]/[NH2;D1;+0:15]>>[C:3]-[#7;a:4]1:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:[c:10](=[O;D1;H0:11]):[n;H0;D3;+0:12]2:[c;H0;D3;+0:1](-[C;D1;H3:2]):[n;H0;D...
91.6
[{"value": 91.0, "product": "CC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 91.6, "product": "CC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
null
null
A mixture of (2Z)-3-pentyl-3,7-dihydro-1H-purine-2,6-dione 2-hydrazone (3.1 g, 0.013 mol) and triethyl orthoacetate (20 mL, 0.1 mol) was heated at 100° C. for 3 h. The suspension was cooled to room temperature and the solid formed was filtered and washed with DCM/Hex (1:1) mixture to provide the desired product (3.1 g,...
10.6084/m9.figshare.5104873.v1
null
Hydrazone.Ether.Ether.Ether
null
c1ncc2nc[nH]c2n1
c1nc2cn3cnnc3nc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
HO-
null
100
null
CCCCCn1/c(=N\N)[nH]c(=O)c2[nH]cnc21.CCOC(C)(OCC)OCC>>CCCCCn1c2nc[nH]c2c(=O)n2c(C)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4afcfa8f3a10469d8d887508de74b55c
CCCCCn1c2nc[nH]c2c(=O)n2c(C)nnc12.O=C1CCC(=O)N1Br>>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(C)nnc12
CC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O.BrN1C(CCC1=O)=O>>BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)C)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([CH3:17])[n:18][n:19][c:20]12.O=C1CCC(=O)N1[Br:10]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([CH3:17])[n:18][n:19][c:20]12
CCCCCn1c2nc[nH]c2c(=O)n2c(C)nnc12.O=C1CCC(=O)N1Br
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(C)nnc12
null
null
C1CCOC1
Functional Group Interconversion
Bromination
ec99ea20e93d70158a8c5b88a0324c2920957b29ee02a6abc4d48c347d7daa1b
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=c1c2[nH]cnc2[nH]c2nncn12
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[cH;D2;+0:9]:[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]>>[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[c;H0;D3;+0:9](-[Br;H0;D1;+0:1]):[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]
31
[{"value": 30.0, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)C)CCCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 31.0, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)C)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
70
CELSIUS
null
null
To a solution of 3-methyl-9-pentyl-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-5-one (1.0 g, 3.8 mmol) in THF (50 mL) was added N-bromosuccinimide (0.75 g, 4.2 mol). The mixture was heated at 70° C. for 1 h and concentrated in vacuum. The residue was taken up in water and EtOAc. The organic layer was separated and the a...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1nc2cn3cnnc3nc2[nH]1.C1CCNC1
c1nc2cn3cnnc3nc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
HO-
C1CCOC1
70
null
CCCCCn1c2nc[nH]c2c(=O)n2c(C)nnc12.O=C1CCC(=O)N1Br>C1CCOC1>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(C)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-41c9da3ea5ee4f24a7ebb47139cdd6e1
CCCCCn1c2nc[nH]c2c(=O)n2c(C)nnc12.O=C1CCC(=O)N1Cl>>CCCCCn1c2nc(Cl)[nH]c2c(=O)n2c(C)nnc12
CC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O.ClN1C(CCC1=O)=O>>ClC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)C)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([CH3:17])[n:18][n:19][c:20]12.O=C1CCC(=O)N1[Cl:10]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Cl:10])[nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([CH3:17])[n:18][n:19][c:20]12
CCCCCn1c2nc[nH]c2c(=O)n2c(C)nnc12.O=C1CCC(=O)N1Cl
CCCCCn1c2nc(Cl)[nH]c2c(=O)n2c(C)nnc12
null
null
C1CCOC1
Functional Group Interconversion
Chlorination
ec99ea20e93d70158a8c5b88a0324c2920957b29ee02a6abc4d48c347d7daa1b
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=c1c2[nH]cnc2[nH]c2nncn12
O=C1-C-C-C(=O)-N-1-[Cl;H0;D1;+0:1].[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[cH;D2;+0:9]:[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]>>[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[c;H0;D3;+0:9](-[Cl;H0;D1;+0:1]):[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]
18.7
[{"value": 18.7, "product": "ClC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)C)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
70
CELSIUS
null
null
To a solution of 3-methyl-9-pentyl-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-5-one (0.10 g, 0.38 mmol) in THF (5 mL) in a microwave reaction tube was added N-chlorosuccinimide (0.046 g, 0.42 mmol). The mixture was heated at 70° C. in a microwave oven for 20 min. After cooling to room temperature, it was purified using...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1nc2cn3cnnc3nc2[nH]1.C1CCNC1
c1nc2cn3cnnc3nc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
HO-
C1CCOC1
70
null
CCCCCn1c2nc[nH]c2c(=O)n2c(C)nnc12.O=C1CCC(=O)N1Cl>C1CCOC1>CCCCCn1c2nc(Cl)[nH]c2c(=O)n2c(C)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b6a78c8703bf436a8f100acc89ee6a82
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.S=C=S>>CCCCCn1c2nc[nH]c2c(=O)n2c(=S)[nH]nc12
C(CCCC)N1/C(/NC(C=2NC=NC12)=O)=N/N.C(=S)=S>>C(CCCC)N1C=2N(C(C=3NC=NC13)=O)C(NN2)=S
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[nH:14]/[c:19]1=[N:18]\[NH2:17].S=[C:15]=[S:16]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[n:14]2[c:15](=[S:16])[nH:17][n:18][c:19]12
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.S=C=S
CCCCCn1c2nc[nH]c2c(=O)n2c(=S)[nH]nc12
null
null
N1=CC=CC=C1
Aromatic Heterocycle Formation
OtherReaction
a709fccbfb10d39ea4751ed4e90ade5fb1f77e1d4eba57b84c8e9008750c73f8
1ce3377721e6f0259a08a7073fbf43200481702e7c26234b4a37d6b14b05ec8b
O=c1c2[nH]cnc2[nH]c2n[nH]c(=S)n12
S=[C;H0;D2;+0:1]=[S;D1;H0:2].[C:3]-[#7;a:4]1:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:[c:10](=[O;D1;H0:11]):[nH;D2;+0:12]/[c;H0;D3;+0:13]:1=[N;H0;D2;+0:14]\[NH2;D1;+0:15]>>[C:3]-[#7;a:4]1:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:[c:10](=[O;D1;H0:11]):[n;H0;D3;+0:12]2:[c;H0;D3;+0:1](=[S;D1;H0:2]):[nH;D2;+0:15]:[n;H0;D2;+0:1...
84.9
[{"value": 84.9, "product": "C(CCCC)N1C=2N(C(C=3NC=NC13)=O)C(NN2)=S", "details": "PERCENTYIELD", "is_desired": false}, {"value": 84.9, "product": "C(CCCC)N1C=2N(C(C=3NC=NC13)=O)C(NN2)=S", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of (2e)-3-pentyl-3,7-dihydro-1h-purine-2,6-dione 2-hydrazone (1.90 g, 8.04 mmol) and carbon disulfide (0.58 ml, 9.64 mmol) in pyridine (30 ml) was stirred at 60° C. for 3 hours. After cooling to room temperature, the solid formed was filtered and dried to yield the desired product (1.90 g, 84.9%). LCMS calcu...
10.6084/m9.figshare.5104873.v1
null
Hydrazone
Thiocarbonyl
c1ncc2nc[nH]c2n1
c1nnc2nc3[nH]cnc3cn12
c1nnc2nc3[nH]cnc3cn12
Other
N1=CC=CC=C1
null
null
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.S=C=S>N1=CC=CC=C1>CCCCCn1c2nc[nH]c2c(=O)n2c(=S)[nH]nc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-866471ddd14747758bb510d78607a3e7
CCCCCn1c2nc[nH]c2c(=O)n2c(=S)[nH]nc12.COS(=O)(=O)OC>>CCCCCn1c2nc[nH]c2c(=O)n2c(SC)nnc12
C(CCCC)N1C=2N(C(C=3NC=NC13)=O)C(NN2)=S.S(=O)(=O)(OC)OC.[OH-].[Na+]>>CSC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[n:14]2[c:15](=[S:16])[nH:18][n:19][c:20]12.COS(=O)(=O)O[CH3:17]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[n:14]2[c:15]([S:16][CH3:17])[n:18][n:19][c:20]12
CCCCCn1c2nc[nH]c2c(=O)n2c(=S)[nH]nc12.COS(=O)(=O)OC
CCCCCn1c2nc[nH]c2c(=O)n2c(SC)nnc12
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
a0d154c906d5fc14b65e6aea6963ae6fb16e5f2f9a94d6135d5a0f3618d8c6f9
e73b6e23c9de2770653dfe1c031448ae08eae1a1e8b31e289bfc4b4719e52064
O=c1c2[nH]cnc2[nH]c2nncn12
C-O-S(=O)(=O)-O-[CH3;D1;+0:1].[#7;a:2]:[c:3]1:[c:4]:[#7;a:5]2:[c:6](:[#7;a:7]:[nH;D2;+0:8]:[c;H0;D3;+0:9]:2=[S;H0;D1;+0:10]):[#7;a:11](-[C:12]):[c:13]:1:[#7;a:14]>>[#7;a:2]:[c:3]1:[c:4]:[#7;a:5]2:[c:6](:[#7;a:7]:[n;H0;D2;+0:8]:[c;H0;D3;+0:9]:2-[S;H0;D2;+0:10]-[CH3;D1;+0:1]):[#7;a:11](-[C:12]):[c:13]:1:[#7;a:14]
85.2
[{"value": 85.2, "product": "CSC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 85.1, "product": "CSC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 9-pentyl-3-thioxo-2,3,6,9-tetrahydro-5h-[1,2,4]triazolo[4,3-a]purin-5-one (1.90 g, 6.83 mmol), dimethyl sulfate (1.03 g, 8.19 mmol) and 1 M of sodium hydroxide in water (25 ml) was stirred at room temperature for 1 hour. The mixture was nutralized to pH=7. The solid formed was filtered and dried to provid...
10.6084/m9.figshare.5104873.v1
null
Thiocarbonyl
Monosulfide
c1nnc2nc3[nH]cnc3cn12
c1nc2cn3cnnc3nc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
HO-
O
null
null
CCCCCn1c2nc[nH]c2c(=O)n2c(=S)[nH]nc12.COS(=O)(=O)OC>O>CCCCCn1c2nc[nH]c2c(=O)n2c(SC)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3f08804eadcd404d816d75c6960834c3
CCCCCn1c2nc[nH]c2c(=O)n2c(SC)nnc12.O=C1CCC(=O)N1Br>>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(SC)nnc12
CSC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O.BrN1C(CCC1=O)=O>>BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)SC)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([S:17][CH3:18])[n:19][n:20][c:21]12.O=C1CCC(=O)N1[Br:10]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([S:17][CH3:18])[n:19][n:20][c:21]12
CCCCCn1c2nc[nH]c2c(=O)n2c(SC)nnc12.O=C1CCC(=O)N1Br
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(SC)nnc12
null
null
O.C1CCOC1
Functional Group Interconversion
Bromination
ec99ea20e93d70158a8c5b88a0324c2920957b29ee02a6abc4d48c347d7daa1b
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=c1c2[nH]cnc2[nH]c2nncn12
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[cH;D2;+0:9]:[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]>>[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[c;H0;D3;+0:9](-[Br;H0;D1;+0:1]):[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]
null
[]
null
null
null
null
A solution of 3-(methylthio)-9-pentyl-6,9-dihydro-5h-[1,2,4]triazolo[4,3-a]purin-5-one (111 mg, 0.380 mmol), N-bromosuccinimide (81.1 mg, 0.456 mmol) in THF (3 ml) was stirred at 70° C. for 3 hours. The reaction was diluted with water and extracted with ethyl acetate three times, dried with sodium sulfate, filtered, an...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1nc2cn3cnnc3nc2[nH]1.C1CCNC1
c1nc2cn3cnnc3nc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
HO-
O.C1CCOC1
null
null
CCCCCn1c2nc[nH]c2c(=O)n2c(SC)nnc12.O=C1CCC(=O)N1Br>O.C1CCOC1>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(SC)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b38acf7db3f4494abf390b4ea925799d
CCCCCn1c2nc[nH]c2c(=O)n2c(S(C)(=O)=O)nnc12.O=C1CCC(=O)N1Br>>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(S(C)=O)nnc12
CS(=O)C1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O.CS(=O)(=O)C1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O.BrN1C(CCC1=O)=O>>BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)S(=O)C)CCCCC
O=[S:17]([c:16]1[n:15]2[c:13](=[O:14])[c:12]3[c:7]([n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:22]2[n:21][n:20]1)[n:8][cH:9][nH:11]3)([CH3:18])=[O:19].O=C1CCC(=O)N1[Br:10]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([S:17]([CH3:18])=[O:19])[n:20][n:21][...
CCCCCn1c2nc[nH]c2c(=O)n2c(S(C)(=O)=O)nnc12.O=C1CCC(=O)N1Br
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(S(C)=O)nnc12
null
null
O.C1CCOC1
Miscellaneous
OtherReaction
6e9a3feacf840bb01f0215e4c654ba2cef799edba173709fc9ea1640b599a3cf
3481437f31f3a5a13cda2b8d72e1defb69168fe81f49152ff712ff76847d3fa7
O=c1c2[nH]cnc2[nH]c2nncn12
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].O=[S;H0;D4;+0:2](-[C;D1;H3:3])(=[O;D1;H0:4])-[c:5]1:[#7;a:6]:[#7;a:7]:[c:8]2:[#7;a:9]:1:[c:10]:[c:11]1:[#7;a:12]:[cH;D2;+0:13]:[#7;a:14]:[c:15]:1:[#7;a:16]:2-[C:17]>>[Br;H0;D1;+0:1]-[c;H0;D3;+0:13]1:[#7;a:12]:[c:11]2:[c:10]:[#7;a:9]3:[c:5](-[S;H0;D3;+0:2](-[C;D1;H3:3])=[O;D1;H0:4]):[#...
null
[]
70
CELSIUS
3
HOUR
To a mixture of 3-(methylsulfinyl)-9-pentyl-6,9-dihydro-5h-[1,2,4]triazolo[4,3-a]purin-5-one and 3-(methylsulfonyl)-9-pentyl-6,9-dihydro-5h-[1,2,4]triazolo[4,3-a]purin-5-one (3:2, 125 mg, 0.40 mmol) in THF (3 mL) was added N-bromosuccinimide (82.3 mg, 0.462 mmol). The mixture was stirred at 70° C. for 3 hours. The reac...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide.Sulfone
Aromatic halide.Sulfoxide
c1nc2cn3cn[nH]c3nc2n1.C1CCNC1
c1nc2cn3cnnc3nc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
HO-
O.C1CCOC1
70
3
CCCCCn1c2nc[nH]c2c(=O)n2c(S(C)(=O)=O)nnc12.O=C1CCC(=O)N1Br>O.C1CCOC1>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(S(C)=O)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f989cf3c6a7f43c89ff1686e63ed6201
CCCCCn1/c(=N\N)[nH]c(=O)c2[nH]cnc21.O=C(n1ccnc1)n1ccnc1>>CCCCCn1c2nc[nH]c2c(=O)n2c(O)nnc12
C(CCCC)N1\C(\NC(C=2NC=NC12)=O)=N/N.C1=CN(C=N1)C(=O)N2C=CN=C2>>OC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[nH:14]/[c:19]1=[N:18]/[NH2:17].c1cn([C:15](n2ccnc2)=[O:16])cn1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[n:14]2[c:15]([OH:16])[n:17][n:18][c:19]12
CCCCCn1/c(=N\N)[nH]c(=O)c2[nH]cnc21.O=C(n1ccnc1)n1ccnc1
CCCCCn1c2nc[nH]c2c(=O)n2c(O)nnc12
null
null
C1CCOC1
Miscellaneous
OtherReaction
e660c8fc9d528787131eca53d54b66bd3a4a3b51061257fd5d3a800307068f7f
0c15633fa8e0570ffdf99d6290e749faeaccbf5a6602f8f904bbba80101d7e4d
O=c1c2[nH]cnc2[nH]c2nncn12
[C:1]-[#7;a:2]1:[c:3]2:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:2:[c:8](=[O;D1;H0:9]):[nH;D2;+0:10]/[c;H0;D3;+0:11]:1=[N;H0;D2;+0:12]/[NH2;D1;+0:13].[O;H0;D1;+0:14]=[C;H0;D3;+0:15](-n1:c:c:n:c:1)-n1:c:c:n:c:1>>[C:1]-[#7;a:2]1:[c:3]2:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:2:[c:8](=[O;D1;H0:9]):[n;H0;D3;+0:10]2:[c;H0;D3;+0:15](-[OH;D1;+0:14...
103.7
[{"value": 98.4, "product": "OC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 103.7, "product": "OC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
null
null
A solution of (2z)-3-pentyl-3,7-dihydro-1h-purine-2,6-dione 2-hydrazone (200 mg, 0.846 mmol), N,N-carbonyldiimidazole (1.65 g, 10.2 mmol) in THF (10 ml) was stirred at 70° C. overnight. The reaction mixture was then heated in microwave reactor at 100° C. for 10 min. The reaction was completed checked by LCMS analysis. ...
10.6084/m9.figshare.5104873.v1
null
Hydrazone
Aromatic alcohol
c1ncc2nc[nH]c2n1.c1c[nH]cn1.c1c[nH]cn1
c1nc2cn3cnnc3nc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
Other
C1CCOC1
100
null
CCCCCn1/c(=N\N)[nH]c(=O)c2[nH]cnc21.O=C(n1ccnc1)n1ccnc1>C1CCOC1>CCCCCn1c2nc[nH]c2c(=O)n2c(O)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9f5ef61842444bd399182df38c7eb900
CCCCCn1c2nc[nH]c2c(=O)n2c(O)nnc12.O=C1CCC(=O)N1Br>>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(O)nnc12
OC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O.BrN1C(CCC1=O)=O>>BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)O)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([OH:17])[n:18][n:19][c:20]12.O=C1CCC(=O)N1[Br:10]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([OH:17])[n:18][n:19][c:20]12
CCCCCn1c2nc[nH]c2c(=O)n2c(O)nnc12.O=C1CCC(=O)N1Br
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(O)nnc12
null
null
C1CCOC1
Functional Group Interconversion
Bromination
ec99ea20e93d70158a8c5b88a0324c2920957b29ee02a6abc4d48c347d7daa1b
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=c1c2[nH]cnc2[nH]c2nncn12
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[cH;D2;+0:9]:[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]>>[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[c;H0;D3;+0:9](-[Br;H0;D1;+0:1]):[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]
null
[]
70
CELSIUS
10
MINUTE
The mixture of solution of 3-hydroxy-9-pentyl-6,9-dihydro-5h-[1,2,4]triazolo[4,3-a]purin-5-one (100 mg, 0.381 mmol) and N-bromosuccinimide (204 mg, 1.14 mmol) in THF (2 ml) was stirred in a microwave reactor at 70° C. for 10 min. The reaction mixture was filtrated and the filtrate was purified by prep LCMS to yield the...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1nc2cn3cnnc3nc2[nH]1.C1CCNC1
c1nc2cn3cnnc3nc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
HO-
C1CCOC1
70
0.166667
CCCCCn1c2nc[nH]c2c(=O)n2c(O)nnc12.O=C1CCC(=O)N1Br>C1CCOC1>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(O)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-17832e53d647405b899d20f820bd49c9
CCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21>>CCCCn1c2nc[nH]c2c(=O)n2cnnc12
C(CCC)N1/C(/NC(C=2NC=NC12)=O)=N/N.C(OCC)([O-])[O-]>>C(CCC)N1C=2N(C(C=3NC=NC13)=O)C=NN2
[CH3:1][CH2:2][CH2:3][CH2:4][n:5]1[c:6]2[n:7][cH:8][nH:9][c:10]2[c:11](=[O:12])[nH:13]/[c:17]1=[N:16]\[NH2:15]>>[CH3:1][CH2:2][CH2:3][CH2:4][n:5]1[c:6]2[n:7][cH:8][nH:9][c:10]2[c:11](=[O:12])[n:13]2[cH:14][n:15][n:16][c:17]12
CCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21
CCCCn1c2nc[nH]c2c(=O)n2cnnc12
null
null
null
Aromatic Heterocycle Formation
OtherReaction
60a3d12ea17afaadb59a56b0f52041f740243ef406a6802686b793ec22e80d0f
d627647f8a5758e4c676083258d3a8813f47848ab7ceb334945a07e482fcef85
O=c1c2[nH]cnc2[nH]c2nncn12
[C:1]-[#7;a:2]1:[c:3]2:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:2:[c:8](=[O;D1;H0:9]):[nH;D2;+0:10]/[c;H0;D3;+0:11]:1=[N;H0;D2;+0:12]\[NH2;D1;+0:13]>>[C:1]-[#7;a:2]1:[c:3]2:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:2:[c:8](=[O;D1;H0:9]):[n;H0;D3;+0:10]2:[c:14]:[n;H0;D2;+0:13]:[n;H0;D2;+0:12]:[c;H0;D3;+0:11]:1:2
71.8
[{"value": 71.8, "product": "C(CCC)N1C=2N(C(C=3NC=NC13)=O)C=NN2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 71.8, "product": "C(CCC)N1C=2N(C(C=3NC=NC13)=O)C=NN2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
null
null
The mixture of (2E)-3-butyl-3,7-dihydro-1H-purine-2,6-dione 2-hydrazone (200 mg, 0.0009 mol) in Ethyl orthoformate (5 mL, 0.03 mol) was heated at 100° C. overnight. After cooling to room temperature, the reaction mixture was filtrated and dried to give the desired product (150 mg, 71.8%). LCMS calculated for C10H13N6O ...
10.6084/m9.figshare.5104873.v1
null
Hydrazone
null
c1ncc2nc[nH]c2n1
c1nc2cn3cnnc3nc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
Other
null
100
null
CCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21>>CCCCn1c2nc[nH]c2c(=O)n2cnnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b140080bbe96414aa828afd3e38d600e
CCCCn1c2nc[nH]c2c(=O)n2cnnc12.O=C1CCC(=O)N1Br>>CCCCn1c2nc(Br)[nH]c2c(=O)n2cnnc12
C(CCC)N1C=2N(C(C=3NC=NC13)=O)C=NN2.BrN1C(CCC1=O)=O>>BrC1=NC=2N(C=3N(C(C2N1)=O)C=NN3)CCCC
[CH3:1][CH2:2][CH2:3][CH2:4][n:5]1[c:6]2[n:7][cH:8][nH:10][c:11]2[c:12](=[O:13])[n:14]2[cH:15][n:16][n:17][c:18]12.O=C1CCC(=O)N1[Br:9]>>[CH3:1][CH2:2][CH2:3][CH2:4][n:5]1[c:6]2[n:7][c:8]([Br:9])[nH:10][c:11]2[c:12](=[O:13])[n:14]2[cH:15][n:16][n:17][c:18]12
CCCCn1c2nc[nH]c2c(=O)n2cnnc12.O=C1CCC(=O)N1Br
CCCCn1c2nc(Br)[nH]c2c(=O)n2cnnc12
null
null
C1CCOC1
Functional Group Interconversion
Bromination
ec99ea20e93d70158a8c5b88a0324c2920957b29ee02a6abc4d48c347d7daa1b
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=c1c2[nH]cnc2[nH]c2nncn12
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[cH;D2;+0:9]:[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]>>[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[c;H0;D3;+0:9](-[Br;H0;D1;+0:1]):[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]
6
[{"value": 6.0, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)C=NN3)CCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 5.5, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)C=NN3)CCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
70
CELSIUS
null
null
To a mixture of 9-butyl-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-5-one (65 mg, 0.28 mmol) in THF (2 mL) was added N-bromosuccinimide (49.8 mg, 0.280 mmol). The mixture was heated in a microwave reactor at 70° C. for 10 minutes. The mixture was purified with prep LCMS to give the desired product (4.8 mg, 6%). LCMS cal...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1nc2cn3cnnc3nc2[nH]1.C1CCNC1
c1nc2cn3cnnc3nc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
HO-
C1CCOC1
70
null
CCCCn1c2nc[nH]c2c(=O)n2cnnc12.O=C1CCC(=O)N1Br>C1CCOC1>CCCCn1c2nc(Br)[nH]c2c(=O)n2cnnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f93cec395f884a94af1db7d40e5ab935
CCCCn1c2nc[nH]c2c(=O)n2c(CCl)nnc12.CO>>CCCCn1c2nc[nH]c2c(=O)n2c(COC)nnc12
C(CCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)CCl.CO>>C(CCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)COC
Cl[CH2:15][c:14]1[n:13]2[c:11](=[O:12])[c:10]3[c:6]([n:5]([CH2:4][CH2:3][CH2:2][CH3:1])[c:20]2[n:19][n:18]1)[n:7][cH:8][nH:9]3.[OH:16][CH3:17]>>[CH3:1][CH2:2][CH2:3][CH2:4][n:5]1[c:6]2[n:7][cH:8][nH:9][c:10]2[c:11](=[O:12])[n:13]2[c:14]([CH2:15][O:16][CH3:17])[n:18][n:19][c:20]12
CCCCn1c2nc[nH]c2c(=O)n2c(CCl)nnc12.CO
CCCCn1c2nc[nH]c2c(=O)n2c(COC)nnc12
null
null
O.C[O-].[Na+]
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
be62d176246b43d48f94f6bacb3beb02bd17fc7ee5c35751334f4a18453b201e
d4b2af534593ebf4ce27dc032f19c2f57b7f68624a1e46dd4bd7343947c883f4
O=c1c2[nH]cnc2[nH]c2nncn12
Cl-[CH2;D2;+0:1]-[c:2]1:[#7;a:3]:[#7;a:4]:[c:5](:[#7;a:6]):[#7;a:7]:1:[c:8]:[c:9]:[#7;a:10].[C;D1;H3:11]-[OH;D1;+0:12]>>[#7;a:6]:[c:5]1:[#7;a:4]:[#7;a:3]:[c:2](-[CH2;D2;+0:1]-[O;H0;D2;+0:12]-[C;D1;H3:11]):[#7;a:7]:1:[c:8]:[c:9]:[#7;a:10]
17.42
[{"value": 17.42, "product": "C(CCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)COC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 1.1, "product": "C(CCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)COC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
The mixture of 9-butyl-3-(chloromethyl)-6,9-dihydro-5h-[1,2,4]triazolo[4,3-a]purin-5-one (35 mg, 125 mmol) in 4 M of sodium methoxide in methanol (0.5 mL, 2 mmol) was stirred at room temperature overnight. The reaction mixture was diluted with water and extracted with ethyl acetate three times. The combined organic lay...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Methanol
Ether
null
null
c1nc2cn3cnnc3nc2[nH]1
HCl
O.C[O-].[Na+]
null
8
CCCCn1c2nc[nH]c2c(=O)n2c(CCl)nnc12.CO>O.C[O-].[Na+]>CCCCn1c2nc[nH]c2c(=O)n2c(COC)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f743fbfcea714bceb87d438a56b30efe
CCCCn1c2nc[nH]c2c(=O)n2c(COC)nnc12.O=C1CCC(=O)N1Br>>CCCCn1c2nc(Br)[nH]c2c(=O)n2c(COC)nnc12
C(CCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)COC.BrN1C(CCC1=O)=O>>BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)COC)CCCC
[CH3:1][CH2:2][CH2:3][CH2:4][n:5]1[c:6]2[n:7][cH:8][nH:10][c:11]2[c:12](=[O:13])[n:14]2[c:15]([CH2:16][O:17][CH3:18])[n:19][n:20][c:21]12.O=C1CCC(=O)N1[Br:9]>>[CH3:1][CH2:2][CH2:3][CH2:4][n:5]1[c:6]2[n:7][c:8]([Br:9])[nH:10][c:11]2[c:12](=[O:13])[n:14]2[c:15]([CH2:16][O:17][CH3:18])[n:19][n:20][c:21]12
CCCCn1c2nc[nH]c2c(=O)n2c(COC)nnc12.O=C1CCC(=O)N1Br
CCCCn1c2nc(Br)[nH]c2c(=O)n2c(COC)nnc12
null
null
O1CCCC1
Functional Group Interconversion
Bromination
ec99ea20e93d70158a8c5b88a0324c2920957b29ee02a6abc4d48c347d7daa1b
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=c1c2[nH]cnc2[nH]c2nncn12
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[cH;D2;+0:9]:[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]>>[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[c;H0;D3;+0:9](-[Br;H0;D1;+0:1]):[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]
null
[]
70
CELSIUS
2
HOUR
The mixture of 9-butyl-3-(methoxymethyl)-6,9-dihydro-5h-[1,2,4]triazolo[4,3-a]purin-5-one (6 mg, 21.7 mmol), N-bromosuccinimide (4.64 mg, 26.0 mmol) in tetrahydrofuran (10 ml) was stirred at 70° C. for 2 hours. The reaction mixture was concentrated in vacuo and the residue was purified by prep LCMS to yield the desired...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1nc2cn3cnnc3nc2[nH]1.C1CCNC1
c1nc2cn3cnnc3nc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
HO-
O1CCCC1
70
2
CCCCn1c2nc[nH]c2c(=O)n2c(COC)nnc12.O=C1CCC(=O)N1Br>O1CCCC1>CCCCn1c2nc(Br)[nH]c2c(=O)n2c(COC)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9f990a135d8f4cf0be48933602f2310c
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=Cc1ccccc1>>CCCCCn1/c(=N/N=Cc2ccccc2)[nH]c(=O)c2[nH]cnc21
C(CCCC)N1/C(/NC(C=2NC=NC12)=O)=N/N.C(C1=CC=CC=C1)=O>>O=C1C=2NC=NC2N(\C(\N1)=N\N=CC1=CC=CC=C1)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1/[c:7](=[N:8]/[NH2:9])[nH:17][c:18](=[O:19])[c:20]2[nH:21][cH:22][n:23][c:24]12.O=[CH:10][c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1/[c:7](=[N:8]/[N:9]=[CH:10][c:11]2[cH:12][cH:13][cH:14][cH:15][cH:16]2)[nH:17][c:18](=[O:19])[c:20]2[nH:...
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=Cc1ccccc1
CCCCCn1/c(=N/N=Cc2ccccc2)[nH]c(=O)c2[nH]cnc21
null
null
C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
369b3f62a39edf615315b2761263eb1b649612c7b3caef083e9b41e01b478de5
a492f13607987389cdd7ab2f9f1199c71d7d1e56ec2df1828d06f8b8bbe23769
O=c1[nH]/c(=N\N=Cc2ccccc2)[nH]c2nc[nH]c12
O=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4].[#7;a:5]/[c:6](=[#7:7]\[NH2;D1;+0:8]):[#7;a:9]>>[#7;a:5]/[c:6](=[#7:7]\[N;H0;D2;+0:8]=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4]):[#7;a:9]
null
[]
null
null
null
null
A solution of (2E)-3-pentyl-3,7-dihydro-1h-purine-2,6-dione 2-hydrazone (104 mg, 44 μmol), benzaldehyde (44.7 μl, 44 μmol) in ethanol (10 ml) was stirred at 70° C. for 3 hours. The reaction solution was concentrated in vacuo to give the desired product. LCMS calculated for C17H21N6O(M+H): 325.2; found: 325.2. Condition...
10.6084/m9.figshare.5104873.v1
null
Hydrazone.Aldehyde
null
null
null
c1ccccc1.c1ncc2[nH]cnc2n1
HO-
C(C)O
null
null
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=Cc1ccccc1>C(C)O>CCCCCn1/c(=N/N=Cc2ccccc2)[nH]c(=O)c2[nH]cnc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-adfed82200a047a3b3a9bd311002b1ca
CCCCCn1/c(=N/N=Cc2ccccc2)[nH]c(=O)c2[nH]cnc21>>CCCCCn1c2nc[nH]c2c(=O)n2c(-c3ccccc3)nnc12
O=C1C=2NC=NC2N(\C(\N1)=N\N=CC1=CC=CC=C1)CCCCC>>C(CCCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)C2=CC=CC=C2
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[nH:14]/[c:24]1=[N:23]\[N:22]=[CH:15][c:16]1[cH:17][cH:18][cH:19][cH:20][cH:21]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[n:14]2[c:15](-[c:16]3[cH:17][cH:18][cH:19][cH:20][cH:21]3)[n:22...
CCCCCn1/c(=N/N=Cc2ccccc2)[nH]c(=O)c2[nH]cnc21
CCCCCn1c2nc[nH]c2c(=O)n2c(-c3ccccc3)nnc12
null
null
C(C)(=O)O
Aromatic Heterocycle Formation
OtherReaction
066077903128dcf5e3d8c17f71c894783195993eb8e78fea83753934f8800b97
42048ba06e684767e79a864f38d2ee087b4547e971032cda3c892dd210eef093
O=c1c2[nH]cnc2[nH]c2nnc(-c3ccccc3)n12
[C:1]-[#7;a:2]1:[c:3]2:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:2:[c:8](=[O;D1;H0:9]):[nH;D2;+0:10]/[c;H0;D3;+0:11]:1=[N;H0;D2;+0:12]\[N;H0;D2;+0:13]=[CH;D2;+0:14]-[c;H0;D3;+0:15](:[c:16]:[c:17]):[c:18]:[c:19]>>[C:1]-[#7;a:2]1:[c:3]2:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:2:[c:8](=[O;D1;H0:9]):[n;H0;D3;+0:10]2:[c;H0;D3;+0:14](-[c;H0;D3;+0...
22
[{"value": 22.0, "product": "C(CCCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)C2=CC=CC=C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 21.5, "product": "C(CCCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)C2=CC=CC=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of benzaldehyde [(2E)-6-oxo-3-pentyl-1,3,6,7-tetrahydro-2h-purin-2-ylidene]hydrazone (140 mg, 0.432 mmol) in acetic acid (5 ml) was stirred at 130° C. for 5 hours. The reaction mixture was concentrated in vacuo and purified by prep LCMS to yield the desired product (30 mg, 22% yield). LCMS calculated for C17...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ncc2nc[nH]c2n1
c1nc2cn3cnnc3nc2[nH]1
c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
null
C(C)(=O)O
null
null
CCCCCn1/c(=N/N=Cc2ccccc2)[nH]c(=O)c2[nH]cnc21>C(C)(=O)O>CCCCCn1c2nc[nH]c2c(=O)n2c(-c3ccccc3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-43868b42f769417590b8eda8ca745004
CCCCCn1c2nc[nH]c2c(=O)n2c(-c3ccccc3)nnc12.O=C1CCC(=O)N1Br>>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(-c3ccccc3)nnc12
C(CCCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)C2=CC=CC=C2.BrN1C(CCC1=O)=O>>BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)C3=CC=CC=C3)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16](-[c:17]3[cH:18][cH:19][cH:20][cH:21][cH:22]3)[n:23][n:24][c:25]12.O=C1CCC(=O)N1[Br:10]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16](-[c:17]3[cH:18][cH:19]...
CCCCCn1c2nc[nH]c2c(=O)n2c(-c3ccccc3)nnc12.O=C1CCC(=O)N1Br
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(-c3ccccc3)nnc12
null
null
C1CCOC1
Functional Group Interconversion
Bromination
ec99ea20e93d70158a8c5b88a0324c2920957b29ee02a6abc4d48c347d7daa1b
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=c1c2[nH]cnc2[nH]c2nnc(-c3ccccc3)n12
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[cH;D2;+0:9]:[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]>>[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[c;H0;D3;+0:9](-[Br;H0;D1;+0:1]):[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]
23.3
[{"value": 23.3, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)C3=CC=CC=C3)CCCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 23.3, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)C3=CC=CC=C3)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
70
CELSIUS
3
HOUR
To a mixture of 9-pentyl-3-phenyl-6,9-dihydro-5h-[1,2,4]triazolo[4,3-a]purin-5-one (30 mg, 0.093 mmol) in THF (30 mL) was added N-bromosuccinimide (19.9 mg, 0.112 mmol). The mixture was stirred at 70° C. for 3 hours. The reaction mixture was concentrated in vacuo and the crude residue was purified using preparative LCM...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1nc2cn3cnnc3nc2[nH]1.C1CCNC1
c1nc2cn3cnnc3nc2[nH]1
c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
HO-
C1CCOC1
70
3
CCCCCn1c2nc[nH]c2c(=O)n2c(-c3ccccc3)nnc12.O=C1CCC(=O)N1Br>C1CCOC1>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(-c3ccccc3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-709c6334c03f4f4fac3a9d5d7fe88588
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(C)nnc12.COc1ccc(CBr)cc1>>CCCCCn1c2nc(Br)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12
BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)C)CCCCC.COC1=CC=C(C=C1)CBr.C([O-])([O-])=O.[K+].[K+]>>BrC1=NC=2N(C=3N(C(C2N1CC1=CC=C(C=C1)OC)=O)C(=NN3)C)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:11][c:21]2[c:22](=[O:23])[n:24]2[c:25]([CH3:26])[n:27][n:28][c:29]12.Br[CH2:12][c:13]1[cH:14][cH:15][c:16]([O:17][CH3:18])[cH:19][cH:20]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[n:11]([CH2:12][c:13]3[cH:14][cH:15][c:16]([O...
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(C)nnc12.COc1ccc(CBr)cc1
CCCCCn1c2nc(Br)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
e7cd22ed9f68e4e320dab4661b2a4d3ee438588eeae829663a94e30f1af40a81
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
O=c1c2c(ncn2Cc2ccccc2)[nH]c2nncn12
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[Br;D1;H0:5]-[c:6]1:[#7;a:7]:[c:8]2:[#7;a:9](-[C:10]):[c:11]3:[#7;a:12]:[#7;a:13]:[c:14]:[#7;a:15]:3:[c:16](=[O;D1;H0:17]):[c:18]:2:[nH;D2;+0:19]:1>>[Br;D1;H0:5]-[c:6]1:[#7;a:7]:[c:8]2:[#7;a:9](-[C:10]):[c:11]3:[#7;a:12]:[#7;a:13]:[c:14]:[#7;a:15]:3:[c:16](=[O;D1;H0:17]):[c:18]:2:[n...
99.7
[{"value": 99.7, "product": "BrC1=NC=2N(C=3N(C(C2N1CC1=CC=C(C=C1)OC)=O)C(=NN3)C)CCCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 99.6, "product": "BrC1=NC=2N(C=3N(C(C2N1CC1=CC=C(C=C1)OC)=O)C(=NN3)C)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
The mixture of 7-bromo-3-methyl-9-pentyl-6,9-dihydro-5h-[1,2,4]triazolo[4,3-a]purin-5-one (200 mg, 0.59 mmol), 4-methoxyphenyl methylbromide (0.094 mL, 0.65 mmol), potassium carbonate (244 mg, 1.77 mmol) in DMF (10 ml) was stirred at room temperature for 2 hours. The reaction was quenched with water and the solid forme...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1nc2cn3cnnc3nc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
HBr
CN(C)C=O
null
2
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(C)nnc12.COc1ccc(CBr)cc1>CN(C)C=O>CCCCCn1c2nc(Br)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6f58e20efc344fccad71273b5fb95504
CCCCCn1c2nc(Br)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12.CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1nccs1>>CCCCCn1c2nc(-c3nccs3)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12
BrC1=NC=2N(C=3N(C(C2N1CC1=CC=C(C=C1)OC)=O)C(=NN3)C)CCCCC.C(CCC)[Sn](C=1SC=CN1)(CCCC)CCCC>>COC1=CC=C(CN2C(=NC=3N(C=4N(C(C23)=O)C(=NN4)C)CCCCC)C=4SC=CN4)C=C1
Br[c:9]1[n:8][c:7]2[n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:33]3[n:28]([c:26](=[O:27])[c:25]2[n:15]1[CH2:16][c:17]1[cH:18][cH:19][c:20]([O:21][CH3:22])[cH:23][cH:24]1)[c:29]([CH3:30])[n:31][n:32]3.CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c:10]1[n:11][cH:12][cH:13][s:14]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8...
CCCCCn1c2nc(Br)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12.CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1nccs1
CCCCCn1c2nc(-c3nccs3)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
C1(=CC=CC=C1)C
C-C Coupling
Stille reaction_aryl
af7798868592fdc1fd977df6782021a84f6e702f80fc2b8d53857a20f289b82e
db27eeefac0475c6d74fa10b3167e95a61caaae74e8bbafd45892452c0c3d4d6
O=c1c2c(nc(-c3nccs3)n2Cc2ccccc2)[nH]c2nncn12
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](:[#7;a:4]):[c:5](:[c:6]:[#7;a:7]):[#7;a:8]:1-[C:9].C-C-C-[CH2]-[Sn](-[CH2]-C-C-C)(-[CH2]-C-C-C)-[c;H0;D3;+0:10]1:[#16;a:11]:[c:12]:[c:13]:[#7;a:14]:1>>[#7;a:7]:[c:6]:[c:5]1:[#7;a:8](-[C:9]):[c;H0;D3;+0:1](-[c;H0;D3;+0:10]2:[#16;a:11]:[c:12]:[c:13]:[#7;a:14]:2):[#7;a:2]:[c:3]:1:[#7;a:4]
79
[{"value": 79.0, "product": "COC1=CC=C(CN2C(=NC=3N(C=4N(C(C23)=O)C(=NN4)C)CCCCC)C=4SC=CN4)C=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 78.4, "product": "COC1=CC=C(CN2C(=NC=3N(C=4N(C(C23)=O)C(=NN4)C)CCCCC)C=4SC=CN4)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To the mixture of 7-bromo-6-(4-methoxybenzyl)-3-methyl-9-pentyl-6,9-dihydro-5h-[1,2,4]triazolo[4,3-a]purin-5-one (100 mg, 0.22 mmol), 2-(tributylstannyl)-1,3-thiazole (122 mg, 0.33 mmol) in toluene (14 mL) was added tetrakis(triphenylphosphine)palladium(0) (12.6 mg, 0.011 mmol) under N2. The mixture was refluxed overni...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Tin
null
c1nc2cn3cnnc3nc2[nH]1.c1cscn1
c1cscn1.c1nc2cn3cnnc3nc2[nH]1
c1cscn1.c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
HBr.Sn
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C1(=CC=CC=C1)C
null
null
CCCCCn1c2nc(Br)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12.CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1nccs1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C1(=CC=CC=C1)C>CCCCCn1c2nc(-c3nccs3)n(Cc3ccc(OC)cc3)c2c(=...
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d0311d2deb804bcfaafef9a3c35fa535
CCCCCn1c2nc(-c3nccs3)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12>>CCCCCn1c2nc(-c3nccs3)[nH]c2c(=O)n2c(C)nnc12
COC1=CC=C(CN2C(=NC=3N(C=4N(C(C23)=O)C(=NN4)C)CCCCC)C=4SC=CN4)C=C1.FC(C(=O)O)(F)F>>CC1=NN=C2N1C(C=1NC(=NC1N2CCCCC)C=2SC=CN2)=O
COc1ccc(C[n:15]2[c:9](-[c:10]3[n:11][cH:12][cH:13][s:14]3)[n:8][c:7]3[n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:24]4[n:19]([c:17](=[O:18])[c:16]32)[c:20]([CH3:21])[n:22][n:23]4)cc1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9](-[c:10]3[n:11][cH:12][cH:13][s:14]3)[nH:15][c:16]2[c:17](=[O:18])[n:19]2[c:20]...
CCCCCn1c2nc(-c3nccs3)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12
CCCCCn1c2nc(-c3nccs3)[nH]c2c(=O)n2c(C)nnc12
null
null
null
Reduction
OtherReaction
6db818c9329237f6c02c4e2815db79463314400b1b8bf7ff3388198d85da62cc
84394d34c591024a84d9393eb3e8adb8ada5a6225c3abafc4dae9aedd4568be4
O=c1c2[nH]c(-c3nccs3)nc2[nH]c2nncn12
C-O-c1:c:c:c(-C-[n;H0;D3;+0:1]2:[c:2]3:[c:3](=[O;D1;H0:4]):[#7;a:5]4:[c:6]:[#7;a:7]:[#7;a:8]:[c:9]:4:[#7;a:10](-[C:11]):[c:12]:3:[#7;a:13]:[c:14]:2-[c:15](:[#16;a:16]):[#7;a:17]):c:c:1>>[#16;a:16]:[c:15](-[c:14]1:[#7;a:13]:[c:12]2:[#7;a:10](-[C:11]):[c:9]3:[#7;a:8]:[#7;a:7]:[c:6]:[#7;a:5]:3:[c:3](=[O;D1;H0:4]):[c:2]:2:...
null
[]
55
CELSIUS
8
HOUR
The mixture of 6-(4-methoxybenzyl)-3-methyl-9-pentyl-7-(1,3-thiazol-2-yl)-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-5-one (100 mg, 0.22 mmol) in trifluoroacetic acid (5 mL, 65 mmol) was stirred at 55° C. overnight. The reaction solution was concentrated and purified using preparative LCMS to yield the desired product....
10.6084/m9.figshare.5104873.v1
null
Ether
null
c1ccccc1.c1nc2nc3nncn3cc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
c1cscn1.c1nc2cn3cnnc3nc2[nH]1
HO-
null
55
8
CCCCCn1c2nc(-c3nccs3)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12>>CCCCCn1c2nc(-c3nccs3)[nH]c2c(=O)n2c(C)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3cf4c7c27a204d9b926be95f1101ac96
CCCCCn1c2nc(Br)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12.CSC>>CCCCCn1c2nc(SC)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12
BrC1=NC=2N(C=3N(C(C2N1CC1=CC=C(C=C1)OC)=O)C(=NN3)C)CCCCC.CSC.[Na].C(OC)COC>>COC1=CC=C(CN2C(=NC=3N(C=4N(C(C23)=O)C(=NN4)C)CCCCC)SC)C=C1
Br[c:9]1[n:8][c:7]2[n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:30]3[n:25]([c:23](=[O:24])[c:22]2[n:12]1[CH2:13][c:14]1[cH:15][cH:16][c:17]([O:18][CH3:19])[cH:20][cH:21]1)[c:26]([CH3:27])[n:28][n:29]3.C[S:10][CH3:11]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([S:10][CH3:11])[n:12]([CH2:13][c:14]3[cH:15]...
CCCCCn1c2nc(Br)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12.CSC
CCCCCn1c2nc(SC)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
5677a31a24a80ab5ae78fbd186bf6c3ddf719007fef37f4369e52ceb2b94f60e
c58e6934d5c82ddec3b0774dc166fdbb9c9ad3acfbb76cde182cbe53c5c1e68c
O=c1c2c(ncn2Cc2ccccc2)[nH]c2nncn12
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](:[#7;a:4]):[c:5](:[c:6]:[#7;a:7]):[#7;a:8]:1-[C:9].C-[S;H0;D2;+0:10]-[C;D1;H3:11]>>[#7;a:7]:[c:6]:[c:5]1:[#7;a:8](-[C:9]):[c;H0;D3;+0:1](-[S;H0;D2;+0:10]-[C;D1;H3:11]):[#7;a:2]:[c:3]:1:[#7;a:4]
79.5
[{"value": 79.5, "product": "COC1=CC=C(CN2C(=NC=3N(C=4N(C(C23)=O)C(=NN4)C)CCCCC)SC)C=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 78.1, "product": "COC1=CC=C(CN2C(=NC=3N(C=4N(C(C23)=O)C(=NN4)C)CCCCC)SC)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 7-bromo-6-(4-methoxybenzyl)-3-methyl-9-pentyl-6,9-dihydro-5h-[1,2,4]triazolo[4,3-a]purin-5-one (271 mg, 0.6 mmol) and sodium methyl sulfide (45.5 mg, 0.65 mmol) in dimethoxyethane (13.4 ml, 129 mmol) was refluxed for 2 h. The reaction was quenched with water. The solid formed was filtered and dried to yiel...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Monosulfide
Monosulfide
c1nc2cn3cnnc3nc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
HBr
null
null
null
CCCCCn1c2nc(Br)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12.CSC>>CCCCCn1c2nc(SC)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-31c63bfb65b549b3bab6aaaa47aade52
CCCCCn1c2nc(SC)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12>>CCCCCn1c2nc(SC)[nH]c2c(=O)n2c(C)nnc12
COC1=CC=C(CN2C(=NC=3N(C=4N(C(C23)=O)C(=NN4)C)CCCCC)SC)C=C1.FC(C(=O)O)(F)F>>CC1=NN=C2N1C(C=1NC(=NC1N2CCCCC)SC)=O
COc1ccc(C[n:12]2[c:9]([S:10][CH3:11])[n:8][c:7]3[n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:21]4[n:16]([c:14](=[O:15])[c:13]32)[c:17]([CH3:18])[n:19][n:20]4)cc1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([S:10][CH3:11])[nH:12][c:13]2[c:14](=[O:15])[n:16]2[c:17]([CH3:18])[n:19][n:20][c:21]12
CCCCCn1c2nc(SC)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12
CCCCCn1c2nc(SC)[nH]c2c(=O)n2c(C)nnc12
null
null
null
Reduction
OtherReaction
6db818c9329237f6c02c4e2815db79463314400b1b8bf7ff3388198d85da62cc
84394d34c591024a84d9393eb3e8adb8ada5a6225c3abafc4dae9aedd4568be4
O=c1c2[nH]cnc2[nH]c2nncn12
C-O-c1:c:c:c(-C-[n;H0;D3;+0:1]2:[c:2]3:[c:3](=[O;D1;H0:4]):[#7;a:5]4:[c:6]:[#7;a:7]:[#7;a:8]:[c:9]:4:[#7;a:10](-[C:11]):[c:12]:3:[#7;a:13]:[c:14]:2-[#16:15]):c:c:1>>[#16:15]-[c:14]1:[#7;a:13]:[c:12]2:[#7;a:10](-[C:11]):[c:9]3:[#7;a:8]:[#7;a:7]:[c:6]:[#7;a:5]:3:[c:3](=[O;D1;H0:4]):[c:2]:2:[nH;D2;+0:1]:1
42
[{"value": 42.0, "product": "CC1=NN=C2N1C(C=1NC(=NC1N2CCCCC)SC)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 0.0, "product": "CC1=NN=C2N1C(C=1NC(=NC1N2CCCCC)SC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 6-(4-methoxybenzyl)-3-methyl-7-(methylthio)-9-pentyl-6,9-dihydro-5h-[1,2,4]triazolo[4,3-a]purin-5-one (200 mg, 469 mmol) in trifluoroacetic acid (5 ml, 64.9 mmol) was stirred at 55° C. overnight. The solution was concentrated and purified by prep LCMS to yield the desired product (60 mg, 42%). 1HNMR (300 ...
10.6084/m9.figshare.5104873.v1
null
Ether
null
c1ccccc1.c1nc2nc3nncn3cc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
HO-
null
null
null
CCCCCn1c2nc(SC)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12>>CCCCCn1c2nc(SC)[nH]c2c(=O)n2c(C)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ac740550c70947df9e901a670c8fae98
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(C)nnc12.OB(O)c1ccccc1>>CCCCCn1c2nc(-c3ccccc3)[nH]c2c(=O)n2c(C)nnc12
BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)C)CCCCC.C1(=CC=CC=C1)B(O)O.C([O-])([O-])=O.[Na+].[Na+]>>CC1=NN=C2N1C(C=1NC(=NC1N2CCCCC)C2=CC=CC=C2)=O
Br[c:9]1[n:8][c:7]2[n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:25]3[n:20]([c:18](=[O:19])[c:17]2[nH:16]1)[c:21]([CH3:22])[n:23][n:24]3.OB(O)[c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9](-[c:10]3[cH:11][cH:12][cH:13][cH:14][cH:15]3)[nH:16][c:17]2[c:18](=[O:19])[n...
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(C)nnc12.OB(O)c1ccccc1
CCCCCn1c2nc(-c3ccccc3)[nH]c2c(=O)n2c(C)nnc12
null
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1
O.COCCOC
C-C Coupling
Suzuki coupling with boronic acids
fba3d7cd2788dca4a8688e3f379e30d3250aa68e83b1dd57d3d04066c5926a02
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=c1c2[nH]c(-c3ccccc3)nc2[nH]c2nncn12
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](:[c:4]:[#7;a:5]):[c:6](:[#7;a:7]):[#7;a:8]:1.O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]>>[#7;a:5]:[c:4]:[c:3]1:[#7;a:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12]:[c:13]):[#7;a:8]:[c:6]:1:[#7;a:7]
16
[{"value": 16.0, "product": "CC1=NN=C2N1C(C=1NC(=NC1N2CCCCC)C2=CC=CC=C2)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 15.9, "product": "CC1=NN=C2N1C(C=1NC(=NC1N2CCCCC)C2=CC=CC=C2)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a mixture of 7-bromo-3-methyl-9-pentyl-6,9-dihydro-5h-[1,2,4]triazolo[4,3-a]purin-5-one (100 mg, 0.30 mmol), phenylboronic acid (39.5 mg, 0.32 mmol), sodium carbonate (100 mg, 0.94 mmol) in water (2 ml) and 1,2-dimethoxyethane (20 ml) was added tetrakis(triphenylphosphine)-palladium(0) (200 mg, 0.10 mmol). The mixtu...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1nc2cn3cnnc3nc2[nH]1.c1ccccc1
c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
HBr.B
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.O.COCCOC
null
null
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(C)nnc12.OB(O)c1ccccc1>[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.O.COCCOC>CCCCCn1c2nc(-c3ccccc3)[nH]c2c(=O)n2c(C)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1d06e169b9be4ce0bc1f293c883e988c
CCCCCn1c2nc(Br)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12.Cn1cc(B2OC(C)(C)C(C)(C)O2)cn1>>CCCCCn1c2nc(-c3cnn(C)c3)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12
BrC1=NC=2N(C=3N(C(C2N1CC1=CC=C(C=C1)OC)=O)C(=NN3)C)CCCCC.CN1N=CC(=C1)B1OC(C(O1)(C)C)(C)C.C([O-])([O-])=O.[Na+].[Na+].C1(=CC=CC=C1)C>>COC1=CC=C(CN2C(=NC=3N(C=4N(C(C23)=O)C(=NN4)C)CCCCC)C=4C=NN(C4)C)C=C1
Br[c:9]1[n:8][c:7]2[n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:34]3[n:29]([c:27](=[O:28])[c:26]2[n:16]1[CH2:17][c:18]1[cH:19][cH:20][c:21]([O:22][CH3:23])[cH:24][cH:25]1)[c:30]([CH3:31])[n:32][n:33]3.CC1(C)OB([c:10]2[cH:11][n:12][n:13]([CH3:14])[cH:15]2)OC1(C)C>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9...
CCCCCn1c2nc(Br)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12.Cn1cc(B2OC(C)(C)C(C)(C)O2)cn1
CCCCCn1c2nc(-c3cnn(C)c3)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
null
C-C Coupling
Suzuki coupling with boronic esters
75a5b19ccbb8196367b85ca33ea640e6be14c6fbbd962b8313a6c4a5baf86024
b42efb3b6a7742d5af594c6a3031e487327e58e9f8c2f428ee68996c98377910
O=c1c2c(nc(-c3cn[nH]c3)n2Cc2ccccc2)[nH]c2nncn12
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](:[#7;a:4]):[c:5](:[c:6]:[#7;a:7]):[#7;a:8]:1-[C:9].C-C1(-C)-O-B(-[c;H0;D3;+0:10]2:[c:11]:[#7;a:12]:[#7;a:13](-[C;D1;H3:14]):[c:15]:2)-O-C-1(-C)-C>>[#7;a:7]:[c:6]:[c:5]1:[#7;a:8](-[C:9]):[c;H0;D3;+0:1](-[c;H0;D3;+0:10]2:[c:11]:[#7;a:12]:[#7;a:13](-[C;D1;H3:14]):[c:15]:2):[#7;a:2]:[c:3]:...
37
[{"value": 37.0, "product": "COC1=CC=C(CN2C(=NC=3N(C=4N(C(C23)=O)C(=NN4)C)CCCCC)C=4C=NN(C4)C)C=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 36.2, "product": "COC1=CC=C(CN2C(=NC=3N(C=4N(C(C23)=O)C(=NN4)C)CCCCC)C=4C=NN(C4)C)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of 7-bromo-6-(4-methoxybenzyl)-3-methyl-9-pentyl-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-5-one (100 mg, 0.3 mmol), 1-methyl-4-(4,4,5,5-tetramethyl-1,3,2-dioxaborolan-2-yl)-1H-pyrazole (92 mg, 0.44 mmol) and sat. sodium carbonate (100 mg, 0.9 mmol) in toluene (20 mL, 0.2 mol) was added tetrakis(tripheny...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic ester
null
c1nc2cn3cnnc3nc2[nH]1.B1OCCO1.c1cn[nH]c1
c1cn[nH]c1.c1nc2cn3cnnc3nc2[nH]1
c1cn[nH]c1.c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
null
null
CCCCCn1c2nc(Br)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12.Cn1cc(B2OC(C)(C)C(C)(C)O2)cn1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1>CCCCCn1c2nc(-c3cnn(C)c3)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5c300066a8d043c1b124fce5af14d968
CCCCCn1c2nc(-c3cnn(C)c3)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12>>CCCCCn1c2nc(-c3cnn(C)c3)[nH]c2c(=O)n2c(C)nnc12
COC1=CC=C(CN2C(=NC=3N(C=4N(C(C23)=O)C(=NN4)C)CCCCC)C=4C=NN(C4)C)C=C1>>CC1=NN=C2N1C(C=1NC(=NC1N2CCCCC)C=2C=NN(C2)C)=O
COc1ccc(C[n:16]2[c:9](-[c:10]3[cH:11][n:12][n:13]([CH3:14])[cH:15]3)[n:8][c:7]3[n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:25]4[n:20]([c:18](=[O:19])[c:17]32)[c:21]([CH3:22])[n:23][n:24]4)cc1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9](-[c:10]3[cH:11][n:12][n:13]([CH3:14])[cH:15]3)[nH:16][c:17]2[c:18](=...
CCCCCn1c2nc(-c3cnn(C)c3)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12
CCCCCn1c2nc(-c3cnn(C)c3)[nH]c2c(=O)n2c(C)nnc12
null
null
FC(C(=O)O)(F)F
Reduction
OtherReaction
6db818c9329237f6c02c4e2815db79463314400b1b8bf7ff3388198d85da62cc
84394d34c591024a84d9393eb3e8adb8ada5a6225c3abafc4dae9aedd4568be4
O=c1c2[nH]c(-c3cn[nH]c3)nc2[nH]c2nncn12
C-O-c1:c:c:c(-C-[n;H0;D3;+0:1]2:[c:2]3:[c:3](=[O;D1;H0:4]):[#7;a:5]4:[c:6]:[#7;a:7]:[#7;a:8]:[c:9]:4:[#7;a:10](-[C:11]):[c:12]:3:[#7;a:13]:[c:14]:2-[c:15]2:[c:16]:[#7;a:17]:[#7;a:18]:[c:19]:2):c:c:1>>[C:11]-[#7;a:10]1:[c:9]2:[#7;a:8]:[#7;a:7]:[c:6]:[#7;a:5]:2:[c:3](=[O;D1;H0:4]):[c:2]2:[nH;D2;+0:1]:[c:14](-[c:15]3:[c:1...
null
[]
null
null
null
null
6-(4-Methoxybenzyl)-3-methyl-7-(1-methyl-1H-pyrazol-4-yl)-9-pentyl-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-5-one (50 mg, 0.10 mmol) in trifluoroacetic acid (5 mL) was stirred at 60° C. overnight. The mixture was concentrated, and the residue was purified by preparative LC-MS to give final product. 1HNMR (300 MHz, CD...
10.6084/m9.figshare.5104873.v1
null
Ether
null
c1ccccc1.c1nc2nc3nncn3cc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
c1cn[nH]c1.c1nc2cn3cnnc3nc2[nH]1
HO-
FC(C(=O)O)(F)F
null
null
CCCCCn1c2nc(-c3cnn(C)c3)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12>FC(C(=O)O)(F)F>CCCCCn1c2nc(-c3cnn(C)c3)[nH]c2c(=O)n2c(C)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b664956537524458a430bb8caaff43a3
CCCCCn1c2nc(Br)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12.c1nc[nH]n1>>CCCCCn1c2nc(-n3cncn3)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12.CCCCCn1c2nc(N3CNC=N3)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12
BrC1=NC=2N(C=3N(C(C2N1CC1=CC=C(C=C1)OC)=O)C(=NN3)C)CCCCC.[H-].[Na+].N1N=CN=C1>>COC1=CC=C(CN2C(=NC=3N(C=4N(C(C23)=O)C(=NN4)C)CCCCC)N4N=CNC4)C=C1.COC1=CC=C(CN2C(=NC=3N(C=4N(C(C23)=O)C(=NN4)C)CCCCC)N4N=CN=C4)C=C1
Br[c:9]1[n:8][c:7]2[n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:33]3[n:28]([c:26](=[O:27])[c:25]2[n:15]1[CH2:49][c:50]1[cH:24][cH:23][c:20]([O:21][CH3:22])[cH:11][cH:51]1)[c:62]([CH3:63])[n:64][n:32]3.[nH:10]1[cH:13][n:12][cH:30][n:14]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9](-[n:10]3[cH:11][n:12][cH...
CCCCCn1c2nc(Br)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12.c1nc[nH]n1
CCCCCn1c2nc(-n3cncn3)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12.CCCCCn1c2nc(N3CNC=N3)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12
null
null
CN(C)C=O
Aromatic Heterocycle Formation
OtherReaction
7a4a6b8b418bffc2cb8dd40f2d479559bcbdc9c46497f03e81a5b6ac97d96017
c4af83b1d37521b1334a837db91c273da1aa79a38a5d4c67440b7a63eb68f111
O=c1c2c(nc(-n3cncn3)n2Cc2ccccc2)[nH]c2nncn12.O=c1c2c(nc(N3CNC=N3)n2Cc2ccccc2)[nH]c2nncn12
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]2:[#7;a:4](-[C:5]):[c:6]3:[n;H0;D2;+0:7]:[n;H0;D2;+0:8]:[c;H0;D3;+0:9](-[C;D1;H3:10]):[n;H0;D3;+0:11]:3:[c:12](=[O;D1;H0:13]):[c:14]:2:[n;H0;D3;+0:15]:1-[CH2;D2;+0:16]-[c;H0;D3;+0:17]1:[cH;D2;+0:18]:[c:19]:[c;H0;D3;+0:20](-[#8:21]-[C;D1;H3:22]):[cH;D2;+0:23]:[cH;D2;+0:24]:1.[cH;D2;+0:25...
27.2
[{"value": 27.2, "product": "COC1=CC=C(CN2C(=NC=3N(C=4N(C(C23)=O)C(=NN4)C)CCCCC)N4N=CNC4)C=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 27.0, "product": "COC1=CC=C(CN2C(=NC=3N(C=4N(C(C23)=O)C(=NN4)C)CCCCC)N4N=CN=C4)C=C1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
Sodium hydride 60% in mineral oil (18 mg, 0.74 mmol) was added to a solution of 1H-1,2,4-Triazole (45 mg, 0.65 mmol) in DMF (10 mL) at room temperature. After stirring for 1 hour at room temperature, 7-bromo-6-(4-methoxybenzyl)-3-methyl-9-pentyl-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-5-one (200 mg, 0.40 mmol) in DM...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ether
Hydrazone.Ether.Ether.Secondary amine
c1ccccc1.c1nc2cn3cnnc3nc2[nH]1.c1nc[nH]n1
c1nc[nH]n1.c1ccccc1.c1nc2cn3cnnc3nc2[nH]1.C1=N[NH]CN1.c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
c1nc[nH]n1.c1ccccc1.c1nc2cn3cnnc3nc2[nH]1.C1=N[NH]CN1.c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
Br-
CN(C)C=O
null
1
CCCCCn1c2nc(Br)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12.c1nc[nH]n1>CN(C)C=O>CCCCCn1c2nc(-n3cncn3)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12.CCCCCn1c2nc(N3CNC=N3)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-cc3352407d79476398c8ef55f2aea4c7
CCCCCn1c2nc(-n3cncn3)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12>>CCCCCn1c2nc(-n3cnnc3)[nH]c2c(=O)n2c(C)nnc12
COC1=CC=C(CN2C(=NC=3N(C=4N(C(C23)=O)C(=NN4)C)CCCCC)N4N=CN=C4)C=C1>>CC1=NN=C2N1C(C=1NC(=NC1N2CCCCC)N2C=NN=C2)=O
COc1ccc(C[n:15]2[c:9](-[n:10]3[cH:11][n:12][cH:14][n:13]3)[n:8][c:7]3[n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:24]4[n:19]([c:17](=[O:18])[c:16]32)[c:20]([CH3:21])[n:22][n:23]4)cc1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9](-[n:10]3[cH:11][n:12][n:13][cH:14]3)[nH:15][c:16]2[c:17](=[O:18])[n:19]2[c:20]...
CCCCCn1c2nc(-n3cncn3)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12
CCCCCn1c2nc(-n3cnnc3)[nH]c2c(=O)n2c(C)nnc12
null
null
FC(C(=O)O)(F)F
Miscellaneous
OtherReaction
9330f0fe78a9d21b6520e542495f5a949884a45542318244a9b5052374ef9304
291cad8b6dfbbd2c823b5c9d45efc37a166dc3454a9f151ac48cb357f4bc155f
O=c1c2[nH]c(-n3cnnc3)nc2[nH]c2nncn12
C-O-c1:c:c:c(-C-[n;H0;D3;+0:1]2:[c:2]3:[c:3](=[O;D1;H0:4]):[#7;a:5]4:[c:6]:[#7;a:7]:[#7;a:8]:[c:9]:4:[#7;a:10](-[C:11]):[c:12]:3:[#7;a:13]:[c:14]:2-[n;H0;D3;+0:15]2:[c:16]:[n;H0;D2;+0:17]:[cH;D2;+0:18]:[n;H0;D2;+0:19]:2):c:c:1>>[C:11]-[#7;a:10]1:[c:9]2:[#7;a:8]:[#7;a:7]:[c:6]:[#7;a:5]:2:[c:3](=[O;D1;H0:4]):[c:2]2:[nH;D...
101.8
[{"value": 52.0, "product": "CC1=NN=C2N1C(C=1NC(=NC1N2CCCCC)N2C=NN=C2)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 101.8, "product": "CC1=NN=C2N1C(C=1NC(=NC1N2CCCCC)N2C=NN=C2)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
8
HOUR
A mixture of 6-(4-methoxybenzyl)-3-methyl-9-pentyl-7-(1H-1,2,4-triazol-1-yl)-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-5-one (53 mg, 0.12 mmol) in trifluoroacetic acid (10 mL) was stirred at 60° C. overnight. The mixture was concentrated and purified by preparative LC-MS to give the desired product (20 mg, 52%). LCMS ...
10.6084/m9.figshare.5104873.v1
null
Ether
null
c1ccccc1.c1nc[nH]n1.c1nc2nc3nncn3cc2[nH]1
c1nnc[nH]1.c1nc2cn3cnnc3nc2[nH]1
c1nnc[nH]1.c1nc2cn3cnnc3nc2[nH]1
HO-
FC(C(=O)O)(F)F
60
8
CCCCCn1c2nc(-n3cncn3)n(Cc3ccc(OC)cc3)c2c(=O)n2c(C)nnc12>FC(C(=O)O)(F)F>CCCCCn1c2nc(-n3cnnc3)[nH]c2c(=O)n2c(C)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-18959035390142b08c14f23249d9e933
CCCCCn1c(N)c(N)c(=O)[nH]c1=S.O=C(O)C1CCC1>>CCCCCn1c(NC(=O)C2CCC2)c(N)c(=O)[nH]c1=S
NC=1C(NC(N(C1N)CCCCC)=S)=O.C1(CCC1)C(=O)O.F[P-](F)(F)(F)(F)F.N1(N=NC2=C1C=CC=C2)O[P+](N(C)C)(N(C)C)N(C)C.C(C)N(CC)CC>>NC1=C(N(C(NC1=O)=S)CCCCC)NC(=O)C1CCC1
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]([NH2:8])[c:15]([NH2:16])[c:17](=[O:18])[nH:19][c:20]1=[S:21].O[C:9](=[O:10])[CH:11]1[CH2:12][CH2:13][CH2:14]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]([NH:8][C:9](=[O:10])[CH:11]2[CH2:12][CH2:13][CH2:14]2)[c:15]([NH2:16])[c:17](=[O:18])[nH:19][c:20]1=[S:21]
CCCCCn1c(N)c(N)c(=O)[nH]c1=S.O=C(O)C1CCC1
CCCCCn1c(NC(=O)C2CCC2)c(N)c(=O)[nH]c1=S
null
null
O.CN(C)C=O
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1cc(=O)[nH]c(=S)[nH]1)C1CCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[C:5].[C:6]-[#7;a:7]1:[c:8]:[#7;a:9]:[c:10]:[c:11]:[c:12]:1-[NH2;D1;+0:13]>>[C:4]-[C:3](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:13]-[c:12]1:[c:11]:[c:10]:[#7;a:9]:[c:8]:[#7;a:7]:1-[C:6])-[C:5]
83.3
[{"value": 83.27, "product": "NC1=C(N(C(NC1=O)=S)CCCCC)NC(=O)C1CCC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 83.3, "product": "NC1=C(N(C(NC1=O)=S)CCCCC)NC(=O)C1CCC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
The mixture of 5,6-diamino-1-pentyl-2-thioxo-2,3-dihydropyrimidin-4(1H)-one (1060 mg, 0.00464 mol), cyclobutane carboxylic acid (0.55 g, 5.5 mmol), benzotriazol-1-yloxytris (dimethylamino)phosphonium hexafluorophosphate (2.2 g, 5.1 mmol) and triethylamine (1.3 mL, 9.3 mmol) in DMF (20 mL) was stirred at room temperatur...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1cncnc1.C1CCC1
HO-
O.CN(C)C=O
null
4
CCCCCn1c(N)c(N)c(=O)[nH]c1=S.O=C(O)C1CCC1>O.CN(C)C=O>CCCCCn1c(NC(=O)C2CCC2)c(N)c(=O)[nH]c1=S
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4db92c15687d4904b441c39586a677c2
CCCCCn1c(NC(=O)C2CCC2)c(N)c(=O)[nH]c1=S>>CCCCCn1c(=S)[nH]c(=O)c2[nH]c(C3CCC3)nc21
NC1=C(N(C(NC1=O)=S)CCCCC)NC(=O)C1CCC1.[OH-].[Na+]>>C1(CCC1)C1=NC=2N(C(NC(C2N1)=O)=S)CCCCC
O=[C:14]([CH:15]1[CH2:16][CH2:17][CH2:18]1)[NH:19][c:20]1[n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:7](=[S:8])[nH:9][c:10](=[O:11])[c:12]1[NH2:13]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7](=[S:8])[nH:9][c:10](=[O:11])[c:12]2[nH:13][c:14]([CH:15]3[CH2:16][CH2:17][CH2:18]3)[n:19][c:20]12
CCCCCn1c(NC(=O)C2CCC2)c(N)c(=O)[nH]c1=S
CCCCCn1c(=S)[nH]c(=O)c2[nH]c(C3CCC3)nc21
null
null
O.CO
Aromatic Heterocycle Formation
OtherReaction
89fa7eaac6a1bd77ac00b2a959bf2d3cfa13bace835949115b1d4cbc9d1a95d8
a079090652d9d6c0e17c70eeab94f6d7afea064f52cf5fa9036d5feedd14143a
O=c1[nH]c(=S)[nH]c2nc(C3CCC3)[nH]c12
O=[C;H0;D3;+0:1](-[NH;D2;+0:2]-[c:3]1:[#7;a:4](-[C:5]):[c:6]:[#7;a:7]:[c:8](=[O;D1;H0:9]):[c:10]:1-[NH2;D1;+0:11])-[C:12](-[C:13])-[C:14]>>[C:13]-[C:12](-[c;H0;D3;+0:1]1:[n;H0;D2;+0:2]:[c:3]2:[#7;a:4](-[C:5]):[c:6]:[#7;a:7]:[c:8](=[O;D1;H0:9]):[c:10]:2:[nH;D2;+0:11]:1)-[C:14]
74.3
[{"value": 73.7, "product": "C1(CCC1)C1=NC=2N(C(NC(C2N1)=O)=S)CCCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 74.3, "product": "C1(CCC1)C1=NC=2N(C(NC(C2N1)=O)=S)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
70
CELSIUS
1
HOUR
The mixture of N-(5-amino-6-oxo-3-pentyl-2-thioxo-1,2,3,6-tetrahydropyrimidin-4-yl)cyclobutanecarboxamide (720 mg, 2.3 mmol) and 2.5 M of sodium hydroxide in water (25 mL) and methanol (25 mL) was stirred at 70° C. for 1 hour. After cooling to room temperature, the reaction mixture was concentrated to remove methanol a...
10.6084/m9.figshare.5104873.v1
null
Secondary amide.Primary amine
null
c1cncnc1
c1ncc2[nH]cnc2n1
c1ncc2[nH]cnc2n1.C1CCC1
HO-
O.CO
70
1
CCCCCn1c(NC(=O)C2CCC2)c(N)c(=O)[nH]c1=S>O.CO>CCCCCn1c(=S)[nH]c(=O)c2[nH]c(C3CCC3)nc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-e83e9624388e4ca09eb26cca5f7fb850
CCCCCn1c(=S)[nH]c(=O)c2[nH]c(C3CCC3)nc21.NN>>CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]c(C3CCC3)nc21
C1(CCC1)C1=NC=2N(C(NC(C2N1)=O)=S)CCCCC.NN>>C1(CCC1)C1=NC=2N(/C(/NC(C2N1)=O)=N/N)CCCCC
S=[c:7]1[n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:21]2[c:13]([c:11](=[O:12])[nH:10]1)[nH:14][c:15]([CH:16]1[CH2:17][CH2:18][CH2:19]1)[n:20]2.[NH2:8][NH2:9]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1/[c:7](=[N:8]/[NH2:9])[nH:10][c:11](=[O:12])[c:13]2[nH:14][c:15]([CH:16]3[CH2:17][CH2:18][CH2:19]3)[n:20][c:21]12
CCCCCn1c(=S)[nH]c(=O)c2[nH]c(C3CCC3)nc21.NN
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]c(C3CCC3)nc21
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
2e80fee15f068129596c03f86e4a84f3567a03df4d28de9eb824e4b8de606d19
b31709867bbae7bd190a95c324309111afc274c1ce2b8bd283fc7d83feae5185
N=c1[nH]c(=O)c2[nH]c(C3CCC3)nc2[nH]1
S=[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4](:[#7;a:5]):[c:6](:[#7;a:7]):[#7;a:8]:1-[C:9].[N;D1;H2:10]-[NH2;D1;+0:11]>>[#7;a:5]:[c:4]1:[c:3]:[#7;a:2]/[c;H0;D3;+0:1](=[N;H0;D2;+0:11]\[N;D1;H2:10]):[#7;a:8](-[C:9]):[c:6]:1:[#7;a:7]
38.6
[{"value": 38.6, "product": "C1(CCC1)C1=NC=2N(/C(/NC(C2N1)=O)=N/N)CCCCC", "details": "PERCENTYIELD", "is_desired": false}]
100
CELSIUS
8
HOUR
The mixture of 8-cyclobutyl-3-pentyl-2-thioxo-1,2,3,7-tetrahydro-6H-purin-6-one (0.6 g, 2.0 mmol) in 20 M of hydrazine in water (20 mL) was stirred at 100° C. overnight. After cooling to room temperature, the solid formed was filtered and dried Cooled down, the solid was isolated to give yield the desired product (230 ...
10.6084/m9.figshare.5104873.v1
null
Hydrazine.Thiocarbonyl
Hydrazone
c1ncc2[nH]cnc2n1
c1ncc2[nH]cnc2n1
c1ncc2[nH]cnc2n1.C1CCC1
Other
O
100
8
CCCCCn1c(=S)[nH]c(=O)c2[nH]c(C3CCC3)nc21.NN>O>CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]c(C3CCC3)nc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-02fce3d897b644f7a805e0f7abcf415d
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]c(C3CCC3)nc21.CCOC(C)(OCC)OCC>>CCCCCn1c2nc(C3CCC3)[nH]c2c(=O)n2c(C)nnc12
C1(CCC1)C1=NC=2N(/C(/NC(C2N1)=O)=N/N)CCCCC.C(C)(OCC)(OCC)OCC>>C1(CCC1)C1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)C)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([CH:10]3[CH2:11][CH2:12][CH2:13]3)[nH:14][c:15]2[c:16](=[O:17])[nH:18]/[c:23]1=[N:22]\[NH2:21].CCO[C:19](OCC)(OCC)[CH3:20]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([CH:10]3[CH2:11][CH2:12][CH2:13]3)[nH:14][c:15]2[c:16](=[O:17])[n:18]2[c:19]([CH...
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]c(C3CCC3)nc21.CCOC(C)(OCC)OCC
CCCCCn1c2nc(C3CCC3)[nH]c2c(=O)n2c(C)nnc12
null
null
null
Aromatic Heterocycle Formation
OtherReaction
ee0085044cada96f0b435a4156edc12d66c02309699c14d468ea3b7289b478ad
d53861995bb64d247d09c3f779c372454b394f82c16bc2582c721d04267c3478
O=c1c2[nH]c(C3CCC3)nc2[nH]c2nncn12
C-C-O-[C;H0;D4;+0:1](-[C;D1;H3:2])(-O-C-C)-O-C-C.[C:3]-[#7;a:4]1:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:[c:10](=[O;D1;H0:11]):[nH;D2;+0:12]/[c;H0;D3;+0:13]:1=[N;H0;D2;+0:14]\[NH2;D1;+0:15]>>[C:3]-[#7;a:4]1:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:2:[c:10](=[O;D1;H0:11]):[n;H0;D3;+0:12]2:[c;H0;D3;+0:1](-[C;D1;H3:2]):[n;H0;D...
10.6
[{"value": 9.2, "product": "C1(CCC1)C1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)C)CCCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 10.6, "product": "C1(CCC1)C1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)C)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
8
HOUR
(2E)-8-cyclobutyl-3-pentyl-3,7-dihydro-1H-purine-2,6-dione 2-hydrazone (100 mg, 0.0003 mol) was mixed with triethyl orthoacetate (10 mL, 0.05 mol) and then stirred at 100° C. overnight. After cooling to room temperature, the mixture was concentrated and purified by preparative LCMS to yield the desired product (10 mg, ...
10.6084/m9.figshare.5104873.v1
null
Hydrazone.Ether.Ether.Ether
null
c1ncc2nc[nH]c2n1
c1nc2cn3cnnc3nc2[nH]1
C1CCC1.c1nc2cn3cnnc3nc2[nH]1
HO-
null
100
8
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]c(C3CCC3)nc21.CCOC(C)(OCC)OCC>>CCCCCn1c2nc(C3CCC3)[nH]c2c(=O)n2c(C)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b4b8f3b3b8e9463da4c1ee9cefd4abea
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.CCN(CC)CC.O=C(O)Cc1ccccc1>>CCCCCn1/c(=N/NC(=O)Cc2ccc(OC)cc2)[nH]c(=O)c2[nH]cnc21
C(CCCC)N1/C(/NC(C=2NC=NC12)=O)=N/N.C1(=CC=CC=C1)CC(=O)O.F[P-](F)(F)(F)(F)F.N1(N=NC2=C1C=CC=C2)O[P+](N(C)C)(N(C)C)N(C)C.C(C)N(CC)CC.CN(C)C=O>>COC1=CC=C(C=C1)CC(=O)N/N=C/1\NC(C=2NC=NC2N1CCCCC)=O
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1/[c:7](=[N:8]/[NH2:9])[nH:21][c:22](=[O:23])[c:24]2[nH:25][cH:26][n:27][c:28]12.CCN(CC)C[CH3:18].[C:10](=[O:11])([CH2:12][c:13]1[cH:14][cH:15][cH:16][cH:19][cH:20]1)[OH:17]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1/[c:7](=[N:8]/[NH:9][C:10](=[O:11])[CH2:12][c:13]2[cH:14][cH:15]...
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.CCN(CC)CC.O=C(O)Cc1ccccc1
CCCCCn1/c(=N/NC(=O)Cc2ccc(OC)cc2)[nH]c(=O)c2[nH]cnc21
null
null
C(C)(=O)OCC
Acylation
OtherReaction
177253170fc482b4e8e53bbe93fc6da9db18600b85c384afc8c6547566a96f38
155f73ccd5cde6fa5b50e1e66b5a06760a53ee9372b42be6acd835f86ba6fca8
O=C(Cc1ccccc1)N/N=c1\[nH]c(=O)c2[nH]cnc2[nH]1
C-C-N(-C-C)-C-[CH3;D1;+0:1].[#7;a:2]/[c:3](=[#7:4]\[NH2;D1;+0:5]):[#7;a:6].[O;D1;H0:7]=[C;H0;D3;+0:8](-[OH;D1;+0:9])-[C:10]-[c:11]1:[c:12]:[c:13]:[cH;D2;+0:14]:[c:15]:[c:16]:1>>[#7;a:2]/[c:3](=[#7:4]\[NH;D2;+0:5]-[C;H0;D3;+0:8](=[O;D1;H0:7])-[C:10]-[c:11]1:[c:12]:[c:13]:[c;H0;D3;+0:14](-[O;H0;D2;+0:9]-[CH3;D1;+0:1]):[c...
98
[{"value": 98.0, "product": "COC1=CC=C(C=C1)CC(=O)N/N=C/1\\NC(C=2NC=NC2N1CCCCC)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
The mixture of (2E)-3-pentyl-3,7-dihydro-1H-purine-2,6-dione 2-hydrazone (0.30 g, 1.3 mmol), benzeneacetic acid, 4-methoxy-(0.23 g, 1.4 mmol), benzotriazol-1-yloxytris-(dimethylamino)phosphonium hexafluorophosphate (0.62 g, 1.40 mmol) and triethylamine (0.53 mL, 3.8 mmol) in DMF (10 mL) were stirred at room temperature...
10.6084/m9.figshare.5104873.v1
null
Hydrazone.Carboxylic acid.Tertiary amine
Hydrazone amide.Ether
c1ccccc1
c1ccccc1
c1ccccc1.c1ncc2[nH]cnc2n1
Other
C(C)(=O)OCC
null
8
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.CCN(CC)CC.O=C(O)Cc1ccccc1>C(C)(=O)OCC>CCCCCn1/c(=N/NC(=O)Cc2ccc(OC)cc2)[nH]c(=O)c2[nH]cnc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ebfc599309aa403ea7c07a239ca90ee4
CCCCCn1/c(=N/NC(=O)Cc2ccc(OC)cc2)[nH]c(=O)c2[nH]cnc21>>CCCCCn1c2nc[nH]c2c(=O)n2c(Cc3ccc(OC)cc3)nnc12
COC1=CC=C(C=C1)CC(=O)N/N=C/1\NC(C=2NC=NC2N1CCCCC)=O>>COC1=CC=C(CC2=NN=C3N2C(C=2NC=NC2N3CCCCC)=O)C=C1
O=[C:15]([CH2:16][c:17]1[cH:18][cH:19][c:20]([O:21][CH3:22])[cH:23][cH:24]1)[NH:25]/[N:26]=[c:27]1/[n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[nH:14]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[n:14]2[c:15]([CH2:16][c:17]3[cH:18]...
CCCCCn1/c(=N/NC(=O)Cc2ccc(OC)cc2)[nH]c(=O)c2[nH]cnc21
CCCCCn1c2nc[nH]c2c(=O)n2c(Cc3ccc(OC)cc3)nnc12
null
null
C1(=CC=CC=C1)C
Aromatic Heterocycle Formation
OtherReaction
f919762557f16e8feb47c1fb62f203cd1ec4ed5f009cf276d2d0e0ec84ef6b80
78b0616e5760c6d4dadfc1fac5c58c0254d0dc7b1bf102fea4bc1349928b0776
O=c1c2[nH]cnc2[nH]c2nnc(Cc3ccccc3)n12
O=[C;H0;D3;+0:1](-[C:2]-[c:3])-[NH;D2;+0:4]/[N;H0;D2;+0:5]=[c;H0;D3;+0:6]1\[nH;D2;+0:7]:[c:8](=[O;D1;H0:9]):[c:10]2:[#7;a:11]:[c:12]:[#7;a:13]:[c:14]:2:[#7;a:15]:1-[C:16]>>[C:16]-[#7;a:15]1:[c:14]2:[#7;a:13]:[c:12]:[#7;a:11]:[c:10]:2:[c:8](=[O;D1;H0:9]):[n;H0;D3;+0:7]2:[c;H0;D3;+0:1](-[C:2]-[c:3]):[n;H0;D2;+0:4]:[n;H0;...
95.5
[{"value": 92.0, "product": "COC1=CC=C(CC2=NN=C3N2C(C=2NC=NC2N3CCCCC)=O)C=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 95.5, "product": "COC1=CC=C(CC2=NN=C3N2C(C=2NC=NC2N3CCCCC)=O)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
The mixture of 2-(4-methoxyphenyl)-N′-[(2E)-6-oxo-3-pentyl-1,3,6,7-tetrahydro-2H-purin-2-ylidene]acetohydrazide (0.66 g, 1.4 mmol) in toluene (30 mL) was refluxed overnight. The reaction mixture was concentrated to give the crude product as a solid. The solid was washed with ethyl acetate and dried to yield the desired...
10.6084/m9.figshare.5104873.v1
null
Hydrazone amide
null
c1ncc2nc[nH]c2n1
c1nc2cn3cnnc3nc2[nH]1
c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
HO-
C1(=CC=CC=C1)C
null
null
CCCCCn1/c(=N/NC(=O)Cc2ccc(OC)cc2)[nH]c(=O)c2[nH]cnc21>C1(=CC=CC=C1)C>CCCCCn1c2nc[nH]c2c(=O)n2c(Cc3ccc(OC)cc3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-31e62738613d44b7b8ed22acef337079
CCCCCn1c2nc[nH]c2c(=O)n2c(Cc3ccc(OC)cc3)nnc12.O=C1CCC(=O)N1Br>>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(Cc3ccc(OC)cc3)nnc12
COC1=CC=C(CC2=NN=C3N2C(C=2NC=NC2N3CCCCC)=O)C=C1.BrN1C(CCC1=O)=O>>BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CC3=CC=C(C=C3)OC)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([CH2:17][c:18]3[cH:19][cH:20][c:21]([O:22][CH3:23])[cH:24][cH:25]3)[n:26][n:27][c:28]12.O=C1CCC(=O)N1[Br:10]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16](...
CCCCCn1c2nc[nH]c2c(=O)n2c(Cc3ccc(OC)cc3)nnc12.O=C1CCC(=O)N1Br
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(Cc3ccc(OC)cc3)nnc12
null
null
C1CCOC1
Functional Group Interconversion
Bromination
ec99ea20e93d70158a8c5b88a0324c2920957b29ee02a6abc4d48c347d7daa1b
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=c1c2[nH]cnc2[nH]c2nnc(Cc3ccccc3)n12
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[cH;D2;+0:9]:[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]>>[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[c;H0;D3;+0:9](-[Br;H0;D1;+0:1]):[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]
60
[{"value": 60.0, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CC3=CC=C(C=C3)OC)CCCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 59.2, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CC3=CC=C(C=C3)OC)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
70
CELSIUS
1
HOUR
To the solution of 3-(4-methoxybenzyl)-9-pentyl-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-5-one (0.40 g, 1.1 mmol) in THF was added N-Bromosuccinimide (0.29 g, 1.6 mmol). The mixture was stirred at 70° C. for 1 hour. The mixture was concentrated and purified by preparative LCMS to yield the desired product (290 mg, 60...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1nc2cn3cnnc3nc2[nH]1.C1CCNC1
c1nc2cn3cnnc3nc2[nH]1
c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
HO-
C1CCOC1
70
1
CCCCCn1c2nc[nH]c2c(=O)n2c(Cc3ccc(OC)cc3)nnc12.O=C1CCC(=O)N1Br>C1CCOC1>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(Cc3ccc(OC)cc3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f9451da4e3474c65a1cbec94728e8aa2
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=C(O)Cc1cccc(Br)c1>>CCCCCn1/c(=N/NC(=O)Cc2cccc(Br)c2)[nH]c(=O)c2[nH]cnc21
C(CCCC)N1/C(/NC(C=2NC=NC12)=O)=N/N.BrC=1C=C(C=CC1)CC(=O)O.F[P-](F)(F)(F)(F)F.N1(N=NC2=C1C=CC=C2)O[P+](N(C)C)(N(C)C)N(C)C.C(C)N(CC)CC>>BrC=1C=C(C=CC1)CC(=O)N/N=C/1\NC(C=2NC=NC2N1CCCCC)=O
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1/[c:7](=[N:8]/[NH2:9])[nH:20][c:21](=[O:22])[c:23]2[nH:24][cH:25][n:26][c:27]12.O[C:10](=[O:11])[CH2:12][c:13]1[cH:14][cH:15][cH:16][c:17]([Br:18])[cH:19]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1/[c:7](=[N:8]/[NH:9][C:10](=[O:11])[CH2:12][c:13]2[cH:14][cH:15][cH:16][c:17]([Br...
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=C(O)Cc1cccc(Br)c1
CCCCCn1/c(=N/NC(=O)Cc2cccc(Br)c2)[nH]c(=O)c2[nH]cnc21
null
null
CN(C)C=O.CCOC(=O)C
Acylation
Carboxylic acid with primary amine to amide
e50d935ef072f0718d4e131af3df793f26e2f0a63884801973739584ab6e55ba
2740512737e2508c1c8d407d0ee271fd1e1c46ad16223e8e2fc1e12936af0dea
O=C(Cc1ccccc1)N/N=c1\[nH]c(=O)c2[nH]cnc2[nH]1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[c:4].[#7;a:5]/[c:6](=[#7:7]\[NH2;D1;+0:8]):[#7;a:9]>>[#7;a:5]/[c:6](=[#7:7]\[NH;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[c:4]):[#7;a:9]
78.2
[{"value": 78.2, "product": "BrC=1C=C(C=CC1)CC(=O)N/N=C/1\\NC(C=2NC=NC2N1CCCCC)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 76.3, "product": "BrC=1C=C(C=CC1)CC(=O)N/N=C/1\\NC(C=2NC=NC2N1CCCCC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
The mixture of (2E)-3-pentyl-3,7-dihydro-1H-purine-2,6-dione 2-hydrazone (0.30 g, 1.3 mmol), (3-bromophenyl)acetic acid (0.30 g, 1.4 mmol), benzotriazol-1-yloxytris-(dimethylamino)phosphonium hexafluorophosphate (0.62 g, 1.4 mol) and triethylamine (0.53 mL, 3.8 mmol) in DMF (10 mL) were stirred at rt overnight. The rea...
10.6084/m9.figshare.5104873.v1
null
Hydrazone.Carboxylic acid
Hydrazone amide
null
null
c1ccccc1.c1ncc2[nH]cnc2n1
HO-
CN(C)C=O.CCOC(=O)C
null
8
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=C(O)Cc1cccc(Br)c1>CN(C)C=O.CCOC(=O)C>CCCCCn1/c(=N/NC(=O)Cc2cccc(Br)c2)[nH]c(=O)c2[nH]cnc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4e5bf53bb28f4121bbf96a56543d181d
CCCCCn1/c(=N/NC(=O)Cc2cccc(Br)c2)[nH]c(=O)c2[nH]cnc21>>CCCCCn1c2nc[nH]c2c(=O)n2c(Cc3cccc(Br)c3)nnc12
BrC=1C=C(C=CC1)CC(=O)N/N=C/1\NC(C=2NC=NC2N1CCCCC)=O>>BrC=1C=C(CC2=NN=C3N2C(C=2NC=NC2N3CCCCC)=O)C=CC1
O=[C:15]([CH2:16][c:17]1[cH:18][cH:19][cH:20][c:21]([Br:22])[cH:23]1)[NH:24]/[N:25]=[c:26]1/[n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[nH:14]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[n:14]2[c:15]([CH2:16][c:17]3[cH:18][cH:19]...
CCCCCn1/c(=N/NC(=O)Cc2cccc(Br)c2)[nH]c(=O)c2[nH]cnc21
CCCCCn1c2nc[nH]c2c(=O)n2c(Cc3cccc(Br)c3)nnc12
null
null
C1=CC=CC=C1
Aromatic Heterocycle Formation
OtherReaction
f919762557f16e8feb47c1fb62f203cd1ec4ed5f009cf276d2d0e0ec84ef6b80
78b0616e5760c6d4dadfc1fac5c58c0254d0dc7b1bf102fea4bc1349928b0776
O=c1c2[nH]cnc2[nH]c2nnc(Cc3ccccc3)n12
O=[C;H0;D3;+0:1](-[C:2]-[c:3])-[NH;D2;+0:4]/[N;H0;D2;+0:5]=[c;H0;D3;+0:6]1\[nH;D2;+0:7]:[c:8](=[O;D1;H0:9]):[c:10]2:[#7;a:11]:[c:12]:[#7;a:13]:[c:14]:2:[#7;a:15]:1-[C:16]>>[C:16]-[#7;a:15]1:[c:14]2:[#7;a:13]:[c:12]:[#7;a:11]:[c:10]:2:[c:8](=[O;D1;H0:9]):[n;H0;D3;+0:7]2:[c;H0;D3;+0:1](-[C:2]-[c:3]):[n;H0;D2;+0:4]:[n;H0;...
86
[{"value": 86.0, "product": "BrC=1C=C(CC2=NN=C3N2C(C=2NC=NC2N3CCCCC)=O)C=CC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
The mixture of 2-(3-bromophenyl)-N′-[(2E)-6-oxo-3-pentyl-1,3,6,7-tetrahydro-2H-purin-2-ylidene]acetohydrazide (1.8 g, 4.2 mmol) in benzene (100 mL) was refluxed overnight. The reaction mixture was concentrated to give the desired product 1.5 g. LCMS calculated for C18H20BrN6O (M+H): 415.1; found: 415.1. Conditions: See...
10.6084/m9.figshare.5104873.v1
null
Hydrazone amide
null
c1ncc2nc[nH]c2n1
c1nc2cn3cnnc3nc2[nH]1
c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
HO-
C1=CC=CC=C1
null
null
CCCCCn1/c(=N/NC(=O)Cc2cccc(Br)c2)[nH]c(=O)c2[nH]cnc21>C1=CC=CC=C1>CCCCCn1c2nc[nH]c2c(=O)n2c(Cc3cccc(Br)c3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-fa37744ffd204ae0bda5eb08decedb0f
CCCCCn1c2nc[nH]c2c(=O)n2c(Cc3cccc(Br)c3)nnc12.O=C1CCC(=O)N1Br>>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(Cc3cccc(Br)c3)nnc12
BrC=1C=C(CC2=NN=C3N2C(C=2NC=NC2N3CCCCC)=O)C=CC1.BrN1C(CCC1=O)=O>>BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CC3=CC(=CC=C3)Br)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([CH2:17][c:18]3[cH:19][cH:20][cH:21][c:22]([Br:23])[cH:24]3)[n:25][n:26][c:27]12.O=C1CCC(=O)N1[Br:10]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([CH2:17...
CCCCCn1c2nc[nH]c2c(=O)n2c(Cc3cccc(Br)c3)nnc12.O=C1CCC(=O)N1Br
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(Cc3cccc(Br)c3)nnc12
null
null
O1CCCC1
Functional Group Interconversion
Bromination
ec99ea20e93d70158a8c5b88a0324c2920957b29ee02a6abc4d48c347d7daa1b
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=c1c2[nH]cnc2[nH]c2nnc(Cc3ccccc3)n12
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[cH;D2;+0:9]:[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]>>[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[c;H0;D3;+0:9](-[Br;H0;D1;+0:1]):[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]
60.7
[{"value": 60.0, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CC3=CC(=CC=C3)Br)CCCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 60.7, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CC3=CC(=CC=C3)Br)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
70
CELSIUS
1
HOUR
To the solution of 3-(3-bromobenzyl)-9-pentyl-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-5-one (210 mg, 0.50 mmol) in tetrahydrofuran (20 mL) was added N-bromosuccinimide (140 mg, 0.00076 mol). The mixture was stirred at 70° C. for 1 hour. The reaction mixture was concentrated and the residue was purified by preparativ...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1nc2cn3cnnc3nc2[nH]1.C1CCNC1
c1nc2cn3cnnc3nc2[nH]1
c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
HO-
O1CCCC1
70
1
CCCCCn1c2nc[nH]c2c(=O)n2c(Cc3cccc(Br)c3)nnc12.O=C1CCC(=O)N1Br>O1CCCC1>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(Cc3cccc(Br)c3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-cc02c5609ee940d09db25e8d72d847db
CCCCCn1/c(=N\N)[nH]c(=O)c2[nH]cnc21.C[N+](C)=C(Cl)Cl>>CCCCCn1c2nc[nH]c2c(=O)n2c(N(C)C)nnc12
[Cl-].ClC(=[N+](C)C)Cl.C(CCCC)N1\C(\NC(C=2NC=NC12)=O)=N/N>>CN(C1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O)C
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[nH:14]/[c:21]1=[N:20]/[NH2:19].Cl[C:15](Cl)=[N+:16]([CH3:17])[CH3:18]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[n:14]2[c:15]([N:16]([CH3:17])[CH3:18])[n:19][n:20][c:21]12
CCCCCn1/c(=N\N)[nH]c(=O)c2[nH]cnc21.C[N+](C)=C(Cl)Cl
CCCCCn1c2nc[nH]c2c(=O)n2c(N(C)C)nnc12
null
null
C(Cl)Cl
Aromatic Heterocycle Formation
OtherReaction
bbdcadb4c7f8309b13790d502223b759d07ee6c6b4a016cb8f5b21ea1012907e
8beb4c10f543b2f2f9ecc23edd744a3451fefe5b77680fd9750f8079fceae275
O=c1c2[nH]cnc2[nH]c2nncn12
Cl-[C;H0;D3;+0:1](-Cl)=[N+;H0;D3:2](-[C;D1;H3:3])-[C;D1;H3:4].[C:5]-[#7;a:6]1:[c:7]2:[#7;a:8]:[c:9]:[#7;a:10]:[c:11]:2:[c:12](=[O;D1;H0:13]):[nH;D2;+0:14]/[c;H0;D3;+0:15]:1=[N;H0;D2;+0:16]/[NH2;D1;+0:17]>>[C:5]-[#7;a:6]1:[c:7]2:[#7;a:8]:[c:9]:[#7;a:10]:[c:11]:2:[c:12](=[O;D1;H0:13]):[n;H0;D3;+0:14]2:[c;H0;D3;+0:1](-[N;...
69.1
[{"value": 69.0, "product": "CN(C1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 69.1, "product": "CN(C1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
5
MINUTE
To methylene chloride (10 mL) was added [B] N-(dichloromethylene)-N-methylmethanaminium chloride (0.21 g, 1.3 mmol). After stirring for 5 mins, (2Z)-3-pentyl-3,7-dihydro-1H-purine-2,6-dione 2-hydrazone (0.10 g, 0.42 mmol) was added, and the mixture was stirred at rt for 5 hrs. LCMS analysis showed product as a major pe...
10.6084/m9.figshare.5104873.v1
null
Hydrazone.Alkenyl halide.Alkenyl halide
Tertiary amine
c1ncc2nc[nH]c2n1
c1nc2cn3cnnc3nc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
HCl
C(Cl)Cl
null
0.083333
CCCCCn1/c(=N\N)[nH]c(=O)c2[nH]cnc21.C[N+](C)=C(Cl)Cl>C(Cl)Cl>CCCCCn1c2nc[nH]c2c(=O)n2c(N(C)C)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a8a45e809d9c4e0aa684e3d357ae4db1
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=C(O)C(F)(F)F>>CCCCCn1c2nc[nH]c2c(=O)n2c(C(F)(F)F)nnc12
C(CCCC)N1/C(/NC(C=2NC=NC12)=O)=N/N.FC(C(=O)O)(F)F>>C(CCCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)C(F)(F)F
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[nH:14]/[c:22]1=[N:21]\[NH2:20].O=[C:15](O)[C:16]([F:17])([F:18])[F:19]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[n:14]2[c:15]([C:16]([F:17])([F:18])[F:19])[n:20][n:21][c:22]12
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=C(O)C(F)(F)F
CCCCCn1c2nc[nH]c2c(=O)n2c(C(F)(F)F)nnc12
null
null
null
Aromatic Heterocycle Formation
OtherReaction
31291cc3561946553fa0a412aac17e231d5f14813122f81265617512be0c5c26
a5b6f2cd9527773fa0ccce3fdf3fdb3e48f4277fe83d66b7b9adab2dd2a35cef
O=c1c2[nH]cnc2[nH]c2nncn12
O-[C;H0;D3;+0:1](=O)-[C:2](-[F;D1;H0:3])(-[F;D1;H0:4])-[F;D1;H0:5].[C:6]-[#7;a:7]1:[c:8]2:[#7;a:9]:[c:10]:[#7;a:11]:[c:12]:2:[c:13](=[O;D1;H0:14]):[nH;D2;+0:15]/[c;H0;D3;+0:16]:1=[N;H0;D2;+0:17]\[NH2;D1;+0:18]>>[C:6]-[#7;a:7]1:[c:8]2:[#7;a:9]:[c:10]:[#7;a:11]:[c:12]:2:[c:13](=[O;D1;H0:14]):[n;H0;D3;+0:15]2:[c;H0;D3;+0:...
60.2
[{"value": 60.2, "product": "C(CCCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)C(F)(F)F", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The mixture of (2E)-3-pentyl-3,7-dihydro-1H-purine-2,6-dione 2-hydrazone (200 mg, 0.85 mmol) in trifluoroacetic acid (10 mL) was refluxed overnight. The reaction mixture was concentrated and purified by preparative LCMS to yield the desired product (160 mg, 60.2%). LCMS calculated for C12H14F3N6O(M+H): 315.1; found 315...
10.6084/m9.figshare.5104873.v1
null
Hydrazone.Carboxylic acid
null
c1ncc2nc[nH]c2n1
c1nc2cn3cnnc3nc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
HO-
null
null
null
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=C(O)C(F)(F)F>>CCCCCn1c2nc[nH]c2c(=O)n2c(C(F)(F)F)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-fe69eed9dcbb4952854932a6a57d0406
CCCCCn1c2nc[nH]c2c(=O)n2c(C(F)(F)F)nnc12.O=C1CCC(=O)N1Br>>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(C(F)(F)F)nnc12
C(CCCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)C(F)(F)F.BrN1C(CCC1=O)=O>>BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)C(F)(F)F)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([C:17]([F:18])([F:19])[F:20])[n:21][n:22][c:23]12.O=C1CCC(=O)N1[Br:10]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([C:17]([F:18])([F:19])[F:20])[n:21][n:...
CCCCCn1c2nc[nH]c2c(=O)n2c(C(F)(F)F)nnc12.O=C1CCC(=O)N1Br
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(C(F)(F)F)nnc12
null
null
O1CCCC1
Functional Group Interconversion
Bromination
ec99ea20e93d70158a8c5b88a0324c2920957b29ee02a6abc4d48c347d7daa1b
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=c1c2[nH]cnc2[nH]c2nncn12
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[cH;D2;+0:9]:[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]>>[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[c;H0;D3;+0:9](-[Br;H0;D1;+0:1]):[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]
null
[]
70
CELSIUS
3
HOUR
To the mixture of 9-pentyl-3-(trifluoromethyl)-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-5-one (50 mg, 0.16 mmol) in tetrahydrofuran (10 mL) was added N-bromosuccinimide (42 mg, 0.24 mmol). The mixture was stirred at 70° C. for 3 hour. The reaction mixture was concentrated and purified by preparative LCMS to yield the...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1nc2cn3cnnc3nc2[nH]1.C1CCNC1
c1nc2cn3cnnc3nc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
HO-
O1CCCC1
70
3
CCCCCn1c2nc[nH]c2c(=O)n2c(C(F)(F)F)nnc12.O=C1CCC(=O)N1Br>O1CCCC1>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(C(F)(F)F)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-38f8855b60e64eb4b4fb666f96d20f37
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21>>CCCCCn1c2nc[nH]c2c(=O)n2nnnc12
N(=O)[O-].[Na+].C(CCCC)N1/C(/NC(C=2NC=NC12)=O)=N/N.C(=O)(O)[O-].[Na+]>>C(CCCC)N1C=2N(C(C=3NC=NC13)=O)N=NN2
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[nH:14]/[c:18]1=[N:17]\[NH2:16]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[n:14]2[n:15][n:16][n:17][c:18]12
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21
CCCCCn1c2nc[nH]c2c(=O)n2nnnc12
null
null
Cl
Aromatic Heterocycle Formation
OtherReaction
4a2d3a022c4e462855afe5b24fdd580fb786023ed6771efe49fffa8dc9f9c8cf
d627647f8a5758e4c676083258d3a8813f47848ab7ceb334945a07e482fcef85
O=c1c2[nH]cnc2[nH]c2nnnn12
[C:1]-[#7;a:2]1:[c:3]2:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:2:[c:8](=[O;D1;H0:9]):[nH;D2;+0:10]/[c;H0;D3;+0:11]:1=[N;H0;D2;+0:12]\[NH2;D1;+0:13]>>[C:1]-[#7;a:2]1:[c:3]2:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:2:[c:8](=[O;D1;H0:9]):[n;H0;D3;+0:10]2:[#7;a:14]:[n;H0;D2;+0:13]:[n;H0;D2;+0:12]:[c;H0;D3;+0:11]:1:2
60.7
[{"value": 60.7, "product": "C(CCCC)N1C=2N(C(C=3NC=NC13)=O)N=NN2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 60.7, "product": "C(CCCC)N1C=2N(C(C=3NC=NC13)=O)N=NN2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A saturated aqueous NaNO2 (130 mg, 1.89 mmol) solution was added dropwise to a solution of (2E)-3-pentyl-3,7-dihydro-1H-purine-2,6-dione 2-hydrazone (150 mg, 0.63 mmol) in 5% aqueous HCl solution (3 ml) under stirring at room temperature. The mixture was stirred at room temperature for 1 hour. The mixture was neutraliz...
10.6084/m9.figshare.5104873.v1
null
Hydrazone
null
c1ncc2nc[nH]c2n1
c1nc2cn3nnnc3nc2[nH]1
c1nc2cn3nnnc3nc2[nH]1
Other
Cl
null
null
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21>Cl>CCCCCn1c2nc[nH]c2c(=O)n2nnnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-51d144eb104145759652ecd78e3a16f8
CCCCCn1c2nc[nH]c2c(=O)n2nnnc12.O=C1CCC(=O)N1Br>>CCCCCn1c2nc(Br)[nH]c2c(=O)n2nnnc12
C(CCCC)N1C=2N(C(C=3NC=NC13)=O)N=NN2.C1CC(=O)N(C1=O)Br>>BrC1=NC=2N(C=3N(C(C2N1)=O)N=NN3)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:11][c:12]2[c:13](=[O:14])[n:15]2[n:16][n:17][n:18][c:19]12.O=C1CCC(=O)N1[Br:10]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:11][c:12]2[c:13](=[O:14])[n:15]2[n:16][n:17][n:18][c:19]12
CCCCCn1c2nc[nH]c2c(=O)n2nnnc12.O=C1CCC(=O)N1Br
CCCCCn1c2nc(Br)[nH]c2c(=O)n2nnnc12
null
null
C1CCOC1
Functional Group Interconversion
Bromination
9d56eb9229def6a6a2150d3c9b0d77729b7e3999fc1a49c972b658a33130521c
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=c1c2[nH]cnc2[nH]c2nnnn12
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[C:2]-[#7;a:3]1:[c:4]2:[#7;a:5]:[#7;a:6]:[#7;a:7]:[#7;a:8]:2:[c:9]:[c:10]2:[#7;a:11]:[cH;D2;+0:12]:[#7;a:13]:[c:14]:1:2>>[Br;H0;D1;+0:1]-[c;H0;D3;+0:12]1:[#7;a:11]:[c:10]2:[c:9]:[#7;a:8]3:[#7;a:7]:[#7;a:6]:[#7;a:5]:[c:4]:3:[#7;a:3](-[C:2]):[c:14]:2:[#7;a:13]:1
13.8
[{"value": 13.7, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)N=NN3)CCCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 13.8, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)N=NN3)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
70
CELSIUS
1
HOUR
The mixture of 4-pentyl-4,7-dihydro-8H-tetrazolo[1,5-a]purin-8-one (94.6 mg, 0.38 mmol) and NBS (75 mg, 0.42 mmol) in THF (20 ml) was stirred at 70° C. for 1 hour. After evaporation of solvent, the residue was purified by preparative LC-MS to yield the desired product (17.1 mg, 13.7%). LCMS calculated for C10H13BrN7O(M...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1nc2cn3nnnc3nc2[nH]1.C1CCNC1
c1nc2cn3nnnc3nc2[nH]1
c1nc2cn3nnnc3nc2[nH]1
HO-
C1CCOC1
70
1
CCCCCn1c2nc[nH]c2c(=O)n2nnnc12.O=C1CCC(=O)N1Br>C1CCOC1>CCCCCn1c2nc(Br)[nH]c2c(=O)n2nnnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a1a59a4f2aa94d2daed7eab7e7570ff3
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=CCCC(=O)O>>CCCCCn1/c(=N/N=C/CCC(=O)O)[nH]c(=O)c2[nH]cnc21
C(CCCC)N1/C(/NC(C=2NC=NC12)=O)=N/N.O=CCCC(=O)O>>O=C1C=2NC=NC2N(\C(\N1)=N\N=C\CCC(=O)O)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1/[c:7](=[N:8]/[NH2:9])[nH:16][c:17](=[O:18])[c:19]2[nH:20][cH:21][n:22][c:23]12.O=[CH:10][CH2:11][CH2:12][C:13](=[O:14])[OH:15]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1/[c:7](=[N:8]/[N:9]=[CH:10]/[CH2:11][CH2:12][C:13](=[O:14])[OH:15])[nH:16][c:17](=[O:18])[c:19]2[nH:20][cH:21...
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=CCCC(=O)O
CCCCCn1/c(=N/N=C/CCC(=O)O)[nH]c(=O)c2[nH]cnc21
null
null
CCO
Heteroatom Alkylation and Arylation
OtherReaction
369b3f62a39edf615315b2761263eb1b649612c7b3caef083e9b41e01b478de5
a492f13607987389cdd7ab2f9f1199c71d7d1e56ec2df1828d06f8b8bbe23769
N=c1[nH]c(=O)c2[nH]cnc2[nH]1
O=[CH;D2;+0:1]-[C:2]-[C:3]-[C:4](=[O;D1;H0:5])-[O;D1;H1:6].[#7;a:7]/[c:8](=[#7:9]\[NH2;D1;+0:10]):[#7;a:11]>>[#7;a:7]/[c:8](=[#7:9]\[N;H0;D2;+0:10]=[CH;D2;+0:1]\[C:2]-[C:3]-[C:4](=[O;D1;H0:5])-[O;D1;H1:6]):[#7;a:11]
96.6
[{"value": 96.0, "product": "O=C1C=2NC=NC2N(\\C(\\N1)=N\\N=C\\CCC(=O)O)CCCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 96.6, "product": "O=C1C=2NC=NC2N(\\C(\\N1)=N\\N=C\\CCC(=O)O)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
The mixture of (2E)-3-pentyl-3,7-dihydro-1H-purine-2,6-dione 2-hydrazone (1.0 g, 4.2 mmol) and 4-oxobutanoic acid (3.4 g, 15% in water, 5.1 mmol) in EtOH (70 ml) was refluxed for 1.5 hours. Evaporation of solvent gave the desired product (1.3 g, 96%) as a yellowish solid. LCMS calculated for C14H21N6O3(M+H): 321.1; fou...
10.6084/m9.figshare.5104873.v1
null
Hydrazone.Aldehyde
null
null
null
c1ncc2[nH]cnc2n1
HO-
CCO
null
null
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=CCCC(=O)O>CCO>CCCCCn1/c(=N/N=C/CCC(=O)O)[nH]c(=O)c2[nH]cnc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-fcaa826f794e409285535240f57be409
CCCCCn1/c(=N/N=C/CCC(=O)O)[nH]c(=O)c2[nH]cnc21>>CCCCCn1c2nc[nH]c2c(=O)n2c(CCC(=O)O)nnc12
O=C1C=2NC=NC2N(\C(\N1)=N\N=C\CCC(=O)O)CCCCC>>O=C1C=2NC=NC2N(C=2N1C(=NN2)CCC(=O)O)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[nH:14]/[c:23]1=[N:22]\[N:21]=[CH:15]\[CH2:16][CH2:17][C:18](=[O:19])[OH:20]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[n:14]2[c:15]([CH2:16][CH2:17][C:18](=[O:19])[OH:20])[n:21][n:22][c:...
CCCCCn1/c(=N/N=C/CCC(=O)O)[nH]c(=O)c2[nH]cnc21
CCCCCn1c2nc[nH]c2c(=O)n2c(CCC(=O)O)nnc12
null
null
C(C)(=O)O
Aromatic Heterocycle Formation
OtherReaction
066077903128dcf5e3d8c17f71c894783195993eb8e78fea83753934f8800b97
42048ba06e684767e79a864f38d2ee087b4547e971032cda3c892dd210eef093
O=c1c2[nH]cnc2[nH]c2nncn12
[C:1]-[#7;a:2]1:[c:3]2:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:2:[c:8](=[O;D1;H0:9]):[nH;D2;+0:10]/[c;H0;D3;+0:11]:1=[N;H0;D2;+0:12]\[N;H0;D2;+0:13]=[CH;D2;+0:14]\[C:15]-[C:16]-[C:17](=[O;D1;H0:18])-[O;D1;H1:19]>>[C:1]-[#7;a:2]1:[c:3]2:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:2:[c:8](=[O;D1;H0:9]):[n;H0;D3;+0:10]2:[c;H0;D3;+0:14](-[C:15]-[...
99
[{"value": 99.0, "product": "O=C1C=2NC=NC2N(C=2N1C(=NN2)CCC(=O)O)CCCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 79.5, "product": "O=C1C=2NC=NC2N(C=2N1C(=NN2)CCC(=O)O)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
The mixture of (4E)-4-[(2E)-(6-oxo-3-pentyl-1,3,6,7-tetrahydro-2H-purin-2-ylidene)hydrazono]butanoic acid (1.367 g, 5.1 mmol) in acetic acid (70 ml) was refluxed for 1 hour. Evaporation of solvent afforded the desired product (1.29 g, 99%) as yellowish solid. LCMS calculated for C14H19N6O3(M+H): 319.2; found: 319.2. Co...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ncc2nc[nH]c2n1
c1nc2cn3cnnc3nc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
null
C(C)(=O)O
null
null
CCCCCn1/c(=N/N=C/CCC(=O)O)[nH]c(=O)c2[nH]cnc21>C(C)(=O)O>CCCCCn1c2nc[nH]c2c(=O)n2c(CCC(=O)O)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f8bce98c4063463ba012f9dc6e29a4d9
CCCCCn1c2nc[nH]c2c(=O)n2c(CCC(=O)O)nnc12.O=C1CCC(=O)N1Br>>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCC(=O)O)nnc12
O=C1C=2NC=NC2N(C=2N1C(=NN2)CCC(=O)O)CCCCC.C1CC(=O)N(C1=O)Br>>BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CCC(=O)O)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([CH2:17][CH2:18][C:19](=[O:20])[OH:21])[n:22][n:23][c:24]12.O=C1CCC(=O)N1[Br:10]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([CH2:17][CH2:18][C:19](=[O:2...
CCCCCn1c2nc[nH]c2c(=O)n2c(CCC(=O)O)nnc12.O=C1CCC(=O)N1Br
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCC(=O)O)nnc12
null
null
C1CCOC1
Functional Group Interconversion
Bromination
ec99ea20e93d70158a8c5b88a0324c2920957b29ee02a6abc4d48c347d7daa1b
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=c1c2[nH]cnc2[nH]c2nncn12
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[cH;D2;+0:9]:[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]>>[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[c;H0;D3;+0:9](-[Br;H0;D1;+0:1]):[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]
23.7
[{"value": 23.7, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CCC(=O)O)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
70
CELSIUS
2
HOUR
The mixture of 3-(5-oxo-9-pentyl-6,9-dihydro-5H[1,2,4]triazolo[4,3-a]purin-3-yl)propanoic acid (203 mg, 0.64 mmole) and NBS (125.8 mg, 7.0 mmol) in THF (25 ml) was stirred at 70° C. for 2 hours. After evaporation of solvent, the residue was purified by preparative LC-MS to afford 60.2 mg (23.7%) of the desired product ...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1nc2cn3cnnc3nc2[nH]1.C1CCNC1
c1nc2cn3cnnc3nc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
HO-
C1CCOC1
70
2
CCCCCn1c2nc[nH]c2c(=O)n2c(CCC(=O)O)nnc12.O=C1CCC(=O)N1Br>C1CCOC1>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCC(=O)O)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-74cc70bfb85842a5b0ee3a6e77d0cdcc
C1COCCN1.CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCC(=O)O)nnc12>>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCC(=O)N3CCOCC3)nnc12
BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CCC(=O)O)CCCCC.N1CCOCC1.C(C)N(CC)CC.F[P-](F)(F)(F)(F)F.N1(N=NC2=C1C=CC=C2)O[P+](N(C)C)(N(C)C)N(C)C>>BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CCC(=O)N3CCOCC3)CCCCC
[NH:21]1[CH2:22][CH2:23][O:24][CH2:25][CH2:26]1.O[C:19]([CH2:18][CH2:17][c:16]1[n:15]2[c:13](=[O:14])[c:12]3[c:7]([n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:29]2[n:28][n:27]1)[n:8][c:9]([Br:10])[nH:11]3)=[O:20]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:1...
C1COCCN1.CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCC(=O)O)nnc12
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCC(=O)N3CCOCC3)nnc12
null
null
C(Cl)Cl
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
2ef483949e7ba3e5f888cf14cdce25fa611f75be09fdf1854a473be519821b59
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C(CCc1nnc2[nH]c3nc[nH]c3c(=O)n12)N1CCOCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4].[#8:5]1-[C:6]-[C:7]-[NH;D2;+0:8]-[C:9]-[C:10]-1>>[C:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[N;H0;D3;+0:8]1-[C:7]-[C:6]-[#8:5]-[C:10]-[C:9]-1
63.3
[{"value": 60.0, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CCC(=O)N3CCOCC3)CCCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 63.3, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CCC(=O)N3CCOCC3)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
The mixture of 3-(7-bromo-5-oxo-9-pentyl-6,9-dihydro-5H[1,2,4]triazolo[4,3-a]purin-3-yl]propanoic acid (50 mg, 0.126 mmol), morpholine (21.0 mg, 0.252 mmol), triethylamine (25.5 mg, 0.252 mmol) and BOP (61.5 mg, 0.139 mmol) in CH2Cl2 (10 ml) was stirred at room temperature for 2 hours. After evaporation of solvent, the...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1COCCN1
C1COCC[NH]1
C1COCC[NH]1.c1nc2cn3cnnc3nc2[nH]1
HO-
C(Cl)Cl
null
2
C1COCCN1.CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCC(=O)O)nnc12>C(Cl)Cl>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCC(=O)N3CCOCC3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d51dd7d15d5e4298aa7b7e63bbb7ea18
N#CCc1ccc(C(F)(F)F)cc1.NO>>N/C(Cc1ccc(C(F)(F)F)cc1)=N\O
FC(C1=CC=C(C=C1)CC#N)(F)F.Cl.NO.C(=O)(O)[O-].[Na+]>>O\N=C(\CC1=CC=C(C=C1)C(F)(F)F)/N
[N:1]#[C:2][CH2:3][c:4]1[cH:5][cH:6][c:7]([C:8]([F:9])([F:10])[F:11])[cH:12][cH:13]1.[NH2:14][OH:15]>>[NH2:1]/[C:2]([CH2:3][c:4]1[cH:5][cH:6][c:7]([C:8]([F:9])([F:10])[F:11])[cH:12][cH:13]1)=[N:14]\[OH:15]
N#CCc1ccc(C(F)(F)F)cc1.NO
N/C(Cc1ccc(C(F)(F)F)cc1)=N\O
null
null
CO
Heteroatom Alkylation and Arylation
Amidoxime from nitrile and hydroxylamine
5f2123b5002b6939ec57e4f55921371a47c78c3ff253c724d87881638fedcd4f
ad3f1127a4d99506976df608684863fb1e08b35faede2d4e31cf4ca96393cd2e
c1ccccc1
[N;H0;D1;+0:1]#[C;H0;D2;+0:2]-[C:3]-[c:4].[NH2;D1;+0:5]-[O;D1;H1:6]>>[NH2;D1;+0:1]/[C;H0;D3;+0:2](-[C:3]-[c:4])=[N;H0;D2;+0:5]\[O;D1;H1:6]
84.9
[{"value": 84.9, "product": "O\\N=C(\\CC1=CC=C(C=C1)C(F)(F)F)/N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 84.9, "product": "O\\N=C(\\CC1=CC=C(C=C1)C(F)(F)F)/N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A suspension of [4-(trifluoromethyl)phenyl]acetonitrile (1.0 g, 5.4 mmoles), hydroxylamine hydrochloride (0.41 g, 5.9 mmoles) and NaHCO3 (0.50 g, 5.9 mmoles) in MeOH (15 ml) was refluxed for 4 hours. The reaction mixture was then concentrated to remove the solvent methanol. The residue was extracted with ethyl acetate....
10.6084/m9.figshare.5104873.v1
null
Nitrile.Primary amine
Primary amine.Oxime
null
null
c1ccccc1
null
CO
null
null
N#CCc1ccc(C(F)(F)F)cc1.NO>CO>N/C(Cc1ccc(C(F)(F)F)cc1)=N\O
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-589a443feaaf49d99d07b72436c20dee
COC(=O)CCC(=O)[O-].N/C(Cc1ccccc1)=N\O>>COC(=O)CCc1nc(Cc2ccccc2)no1
C(CCC(=O)[O-])(=O)OC.C1=CN(C=N1)C(=O)N2C=CN=C2.O\N=C(\CC1=CC=CC=C1)/N>>C(C1=CC=CC=C1)C1=NOC(=N1)CCC(=O)OC
O=[C:7]([O-])[CH2:6][CH2:5][C:3]([O:2][CH3:1])=[O:4].[NH2:8]/[C:9]([CH2:10][c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1)=[N:17]\[OH:18]>>[CH3:1][O:2][C:3](=[O:4])[CH2:5][CH2:6][c:7]1[n:8][c:9]([CH2:10][c:11]2[cH:12][cH:13][cH:14][cH:15][cH:16]2)[n:17][o:18]1
COC(=O)CCC(=O)[O-].N/C(Cc1ccccc1)=N\O
COC(=O)CCc1nc(Cc2ccccc2)no1
null
null
CN(C)C=O
Aromatic Heterocycle Formation
OtherReaction
d5c6320841f1ab27aeecb31a475839e66def5aa9eb9bb79c83570ae0a04a0046
e4d0a49bc358c8febd1a5e454066b0a955c97759f5381ecc96c210781772c661
c1ccc(Cc2ncon2)cc1
O=[C;H0;D3;+0:1](-[O-])-[C:2]-[C:3]-[C:4](-[#8:5])=[O;D1;H0:6].[NH2;D1;+0:7]/[C;H0;D3;+0:8](-[C:9]-[c:10])=[N;H0;D2;+0:11]\[OH;D1;+0:12]>>[#8:5]-[C:4](=[O;D1;H0:6])-[C:3]-[C:2]-[c;H0;D3;+0:1]1:[n;H0;D2;+0:7]:[c;H0;D3;+0:8](-[C:9]-[c:10]):[n;H0;D2;+0:11]:[o;H0;D2;+0:12]:1
69.7
[{"value": 69.7, "product": "C(C1=CC=CC=C1)C1=NOC(=N1)CCC(=O)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 69.7, "product": "C(C1=CC=CC=C1)C1=NOC(=N1)CCC(=O)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
Butanedioic acid, monomethyl ester (4.0 g, 30.3 mmole) and CDI (5.40 g, 33.3 mmole) were dissolved in anhydrous DMF (15 ml). After stirring the solution at room temperature for 3 hours, (1Z)-N′-hydroxy-2-phenylethanimidamide (5.0 g, 33.3 mmole) was added and the solution heated at 90° C. for 20 hours. After evaporation...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Oxime
null
null
c1ncon1
c1ncon1.c1ccccc1
HO-
CN(C)C=O
null
3
COC(=O)CCC(=O)[O-].N/C(Cc1ccccc1)=N\O>CN(C)C=O>COC(=O)CCc1nc(Cc2ccccc2)no1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-aa85ff1308584931b01fcd4382dc7026
COC(=O)CCc1nc(Cc2ccccc2)no1>>O=C(O)CCc1nc(Cc2ccccc2)no1
C(C1=CC=CC=C1)C1=NOC(=N1)CCC(=O)OC.[OH-].[Na+]>>C(C1=CC=CC=C1)C1=NOC(=N1)CCC(=O)O
C[O:3][C:2](=[O:1])[CH2:4][CH2:5][c:6]1[n:7][c:8]([CH2:9][c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[n:16][o:17]1>>[O:1]=[C:2]([OH:3])[CH2:4][CH2:5][c:6]1[n:7][c:8]([CH2:9][c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[n:16][o:17]1
COC(=O)CCc1nc(Cc2ccccc2)no1
O=C(O)CCc1nc(Cc2ccccc2)no1
null
null
CO
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(Cc2ncon2)cc1
C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
98
[{"value": 98.0, "product": "C(C1=CC=CC=C1)C1=NOC(=N1)CCC(=O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 98.0, "product": "C(C1=CC=CC=C1)C1=NOC(=N1)CCC(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
To a solution of methyl 3-(3-benzyl-1,2,4-oxadiazol-5-yl)propanoate (5.2 g, 21.1 mmole) in methanol (30 ml) was added 50 ml of 1N NaOH. The mixture was stirred at room temperature for 2 hours. The mixture was adjusted to PH=3-4 under ice bath, and extracted with EtOAc (3×). The combined organic phases were washed with ...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ncon1.c1ccccc1
Other
CO
null
2
COC(=O)CCc1nc(Cc2ccccc2)no1>CO>O=C(O)CCc1nc(Cc2ccccc2)no1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-821af4ae7034437e9f13426e6590559d
CCCCCn1/c(=N/NC(=O)CCc2nc(Cc3ccccc3)no2)[nH]c(=O)c2[nH]c(C(F)(F)F)nc21>>CCCCCn1c2nc(C(F)(F)F)[nH]c2c(=O)n2c(CCc3nc(Cc4ccccc4)no3)nnc12
C(C1=CC=CC=C1)C1=NOC(=N1)CCC(=O)N/N=C/1\NC(C=2NC(=NC2N1CCCCC)C(F)(F)F)=O>>C(C1=CC=CC=C1)C1=NOC(=N1)CCC1=NN=C2N1C(C=1NC(=NC1N2CCCCC)C(F)(F)F)=O
O=[C:19]([CH2:20][CH2:21][c:22]1[n:23][c:24]([CH2:25][c:26]2[cH:27][cH:28][cH:29][cH:30][cH:31]2)[n:32][o:33]1)[NH:34]/[N:35]=[c:36]1/[n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:7]2[n:8][c:9]([C:10]([F:11])([F:12])[F:13])[nH:14][c:15]2[c:16](=[O:17])[nH:18]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([...
CCCCCn1/c(=N/NC(=O)CCc2nc(Cc3ccccc3)no2)[nH]c(=O)c2[nH]c(C(F)(F)F)nc21
CCCCCn1c2nc(C(F)(F)F)[nH]c2c(=O)n2c(CCc3nc(Cc4ccccc4)no3)nnc12
null
null
C1(=CC=CC=C1)C
Aromatic Heterocycle Formation
OtherReaction
f919762557f16e8feb47c1fb62f203cd1ec4ed5f009cf276d2d0e0ec84ef6b80
78b0616e5760c6d4dadfc1fac5c58c0254d0dc7b1bf102fea4bc1349928b0776
O=c1c2[nH]cnc2[nH]c2nnc(CCc3nc(Cc4ccccc4)no3)n12
O=[C;H0;D3;+0:1](-[C:2]-[C:3])-[NH;D2;+0:4]/[N;H0;D2;+0:5]=[c;H0;D3;+0:6]1\[nH;D2;+0:7]:[c:8](=[O;D1;H0:9]):[c:10]2:[#7;a:11]:[c:12]:[#7;a:13]:[c:14]:2:[#7;a:15]:1-[C:16]>>[C:3]-[C:2]-[c;H0;D3;+0:1]1:[n;H0;D2;+0:4]:[n;H0;D2;+0:5]:[c;H0;D3;+0:6]2:[#7;a:15](-[C:16]):[c:14]3:[#7;a:13]:[c:12]:[#7;a:11]:[c:10]:3:[c:8](=[O;D...
17.9
[{"value": 17.8, "product": "C(C1=CC=CC=C1)C1=NOC(=N1)CCC1=NN=C2N1C(C=1NC(=NC1N2CCCCC)C(F)(F)F)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 17.9, "product": "C(C1=CC=CC=C1)C1=NOC(=N1)CCC1=NN=C2N1C(C=1NC(=NC1N2CCCCC)C(F)(F)F)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
The mixture of 3-(3-benzyl-1,2,4-oxadiazol-5-yl)-N′-[(2E)-6-oxo-3-pentyl-8-(trifluoromethyl)-1,3,6,7-tetrahydro-2H-purin-2-ylidene]propanohydrazide (220.1 mg, 0.424 mmole) in toluene (20 ml) was refluxed for 5 hours. After evaporation of solvent, the residue was purified by preparative LCMS to yield the desired product...
10.6084/m9.figshare.5104873.v1
null
Hydrazone amide
null
c1ncc2nc[nH]c2n1
c1nc2cn3cnnc3nc2[nH]1
c1ncon1.c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
HO-
C1(=CC=CC=C1)C
null
null
CCCCCn1/c(=N/NC(=O)CCc2nc(Cc3ccccc3)no2)[nH]c(=O)c2[nH]c(C(F)(F)F)nc21>C1(=CC=CC=C1)C>CCCCCn1c2nc(C(F)(F)F)[nH]c2c(=O)n2c(CCc3nc(Cc4ccccc4)no3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-3805461a52d641f885f11aa035677179
COC(=O)CCC(=O)[O-].NNC(=O)c1ccccc1>>COC(=O)CCC(=O)NNC(=O)c1ccccc1
C(C1=CC=CC=C1)(=O)NN.C(CCC(=O)[O-])(=O)OC.F[P-](F)(F)(F)(F)F.N1(N=NC2=C1C=CC=C2)O[P+](N(C)C)(N(C)C)N(C)C.C(C)(C)N(C(C)C)CC>>C(C1=CC=CC=C1)(=O)NNC(CCC(=O)OC)=O
[O-][C:7]([CH2:6][CH2:5][C:3]([O:2][CH3:1])=[O:4])=[O:8].[NH2:9][NH:10][C:11](=[O:12])[c:13]1[cH:14][cH:15][cH:16][cH:17][cH:18]1>>[CH3:1][O:2][C:3](=[O:4])[CH2:5][CH2:6][C:7](=[O:8])[NH:9][NH:10][C:11](=[O:12])[c:13]1[cH:14][cH:15][cH:16][cH:17][cH:18]1
COC(=O)CCC(=O)[O-].NNC(=O)c1ccccc1
COC(=O)CCC(=O)NNC(=O)c1ccccc1
null
CN(C1=CC=NC=C1)C
CN(C)C=O
Acylation
OtherReaction
84d993f2dd8c5d113c44b49ecd8621492b66c5d2b94f73a7d5ff99800e371df5
b956b8a4acbeafca0fa5a0ba87177355a422ec6427e7d47cc2545547616c0ab5
c1ccccc1
[#8:1]-[C:2](=[O;D1;H0:3])-[C:4]-[C:5]-[C;H0;D3;+0:6](-[O-])=[O;D1;H0:7].[NH2;D1;+0:8]-[#7:9]-[C:10](=[O;D1;H0:11])-[c:12]>>[#8:1]-[C:2](=[O;D1;H0:3])-[C:4]-[C:5]-[C;H0;D3;+0:6](=[O;D1;H0:7])-[NH;D2;+0:8]-[#7:9]-[C:10](=[O;D1;H0:11])-[c:12]
32.7
[{"value": 32.6, "product": "C(C1=CC=CC=C1)(=O)NNC(CCC(=O)OC)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 32.7, "product": "C(C1=CC=CC=C1)(=O)NNC(CCC(=O)OC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
The mixture of benzhydrazide (1.5 g, 11.0 mmol), butanedioic acid, monomethyl ester (2.0 g, 15 mmol), benzotriazol-1-yloxytris(dimethylamino)phosphonium hexafluorophosphate (5.4 g, 12 mmol), N,N-diisopropylethylamine (3.8 mL, 22 mmol) and 4-dimethylaminopyridine (0.87 g, 7.2 mmol) in DMF (30 mL) was stirred at room tem...
10.6084/m9.figshare.5104873.v1
null
Acylhydrazine
Acylhydrazine.Acylhydrazine
null
null
c1ccccc1
HO-
CN(C1=CC=NC=C1)C.CN(C)C=O
null
8
COC(=O)CCC(=O)[O-].NNC(=O)c1ccccc1>CN(C1=CC=NC=C1)C.CN(C)C=O>COC(=O)CCC(=O)NNC(=O)c1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-76b0c845b0fb4a93891c0a3157acf0dd
COC(=O)CCC(=O)NNC(=O)c1ccccc1>>COC(=O)CCc1nnc(-c2ccccc2)o1
S(=O)(Cl)Cl.C(C1=CC=CC=C1)(=O)NNC(CCC(=O)OC)=O.N1=CC=CC=C1>>C1(=CC=CC=C1)C1=NN=C(O1)CCC(=O)OC
O=[C:7]([CH2:6][CH2:5][C:3]([O:2][CH3:1])=[O:4])[NH:8][NH:9][C:10]([c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1)=[O:17]>>[CH3:1][O:2][C:3](=[O:4])[CH2:5][CH2:6][c:7]1[n:8][n:9][c:10](-[c:11]2[cH:12][cH:13][cH:14][cH:15][cH:16]2)[o:17]1
COC(=O)CCC(=O)NNC(=O)c1ccccc1
COC(=O)CCc1nnc(-c2ccccc2)o1
null
null
O1CCCC1
Aromatic Heterocycle Formation
OtherReaction
ef130645674b014a808ae327ff67ae63a4b0fba1781fc176f61089abd6ffd017
b3d4fa0dcfa02ac7642075a89f830594ba71dc7452e661900a986719bd6ddb0a
c1ccc(-c2nnco2)cc1
O=[C;H0;D3;+0:1](-[C:2]-[C:3]-[C:4](-[#8:5])=[O;D1;H0:6])-[NH;D2;+0:7]-[NH;D2;+0:8]-[C;H0;D3;+0:9](=[O;H0;D1;+0:10])-[c;H0;D3;+0:11](:[c:12]:[c:13]):[c:14]:[c:15]>>[#8:5]-[C:4](=[O;D1;H0:6])-[C:3]-[C:2]-[c;H0;D3;+0:1]1:[n;H0;D2;+0:7]:[n;H0;D2;+0:8]:[c;H0;D3;+0:9](-[c;H0;D3;+0:11](:[c:12]:[c:13]):[c:14]:[c:15]):[o;H0;D2...
72
[{"value": 72.0, "product": "C1(=CC=CC=C1)C1=NN=C(O1)CCC(=O)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 64.6, "product": "C1(=CC=CC=C1)C1=NN=C(O1)CCC(=O)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
Thionyl chloride (0.34 mL, 4.7 mmol) was added to the mixture of methyl 4-(2-benzoylhydrazino)-4-oxobutanoate (900 mg, 4 mmol), Pyridine (0.87 mL, 0.011 mol) in tetrahydrofuran (20 mL) at room temperature. After stirring for 3 hours, the reaction mixture was concentrated. The residue was mixed with toluene (20 mL) and ...
10.6084/m9.figshare.5104873.v1
null
Acylhydrazine.Acylhydrazine
null
null
c1nnco1
c1nnco1.c1ccccc1
HO-
O1CCCC1
null
3
COC(=O)CCC(=O)NNC(=O)c1ccccc1>O1CCCC1>COC(=O)CCc1nnc(-c2ccccc2)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7346673dc2d34e998c69654afd855478
COC(=O)CCc1nnc(-c2ccccc2)o1>>O=C(O)CCc1nnc(-c2ccccc2)o1
C1(=CC=CC=C1)C1=NN=C(O1)CCC(=O)OC>>C1(=CC=CC=C1)C1=NN=C(O1)CCC(=O)O
C[O:3][C:2](=[O:1])[CH2:4][CH2:5][c:6]1[n:7][n:8][c:9](-[c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[o:16]1>>[O:1]=[C:2]([OH:3])[CH2:4][CH2:5][c:6]1[n:7][n:8][c:9](-[c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[o:16]1
COC(=O)CCc1nnc(-c2ccccc2)o1
O=C(O)CCc1nnc(-c2ccccc2)o1
null
null
CO.[OH-].[Na+]
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(-c2nnco2)cc1
C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
114.6
[{"value": 83.0, "product": "C1(=CC=CC=C1)C1=NN=C(O1)CCC(=O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 114.6, "product": "C1(=CC=CC=C1)C1=NN=C(O1)CCC(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
A mixture of methyl 3-(5-phenyl-1,3,4-oxadiazol-2-yl)propanoate (600 mg, 2.0 mmol) in 1 M of aqueous NaOH (10 mL) and Methanol (10 mL) was stirred at room temperature overnight. The reaction solution was adjusted to pH 5 and extracted with ethyl acetate three times. The combined organic layers were dried, filtered and ...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1nnco1.c1ccccc1
Other
CO.[OH-].[Na+]
null
8
COC(=O)CCc1nnc(-c2ccccc2)o1>CO.[OH-].[Na+]>O=C(O)CCc1nnc(-c2ccccc2)o1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0f318cc8935a474185eba9878b8756d9
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=C(O)CCc1nnc(-c2ccccc2)o1>>CCCCCn1/c(=N/NC(=O)CCc2nnc(-c3ccccc3)o2)[nH]c(=O)c2[nH]cnc21
C1(=CC=CC=C1)C1=NN=C(O1)CCC(=O)O.C(CCCC)N1/C(/NC(C=2NC=NC12)=O)=N/N.F[P-](F)(F)(F)(F)F.N1(N=NC2=C1C=CC=C2)O[P+](N(C)C)(N(C)C)N(C)C.C(C)(C)N(C(C)C)CC>>O=C1C=2NC=NC2N(\C(\N1)=N\NC(CCC=1OC(=NN1)C1=CC=CC=C1)=O)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1/[c:7](=[N:8]/[NH2:9])[nH:25][c:26](=[O:27])[c:28]2[nH:29][cH:30][n:31][c:32]12.O[C:10](=[O:11])[CH2:12][CH2:13][c:14]1[n:15][n:16][c:17](-[c:18]2[cH:19][cH:20][cH:21][cH:22][cH:23]2)[o:24]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1/[c:7](=[N:8]/[NH:9][C:10](=[O:11])[CH2:12][CH...
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=C(O)CCc1nnc(-c2ccccc2)o1
CCCCCn1/c(=N/NC(=O)CCc2nnc(-c3ccccc3)o2)[nH]c(=O)c2[nH]cnc21
null
CN(C1=CC=NC=C1)C
CN(C)C=O
Acylation
Carboxylic acid with primary amine to amide
e50d935ef072f0718d4e131af3df793f26e2f0a63884801973739584ab6e55ba
2740512737e2508c1c8d407d0ee271fd1e1c46ad16223e8e2fc1e12936af0dea
O=C(CCc1nnc(-c2ccccc2)o1)N/N=c1\[nH]c(=O)c2[nH]cnc2[nH]1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4].[#7;a:5]/[c:6](=[#7:7]\[NH2;D1;+0:8]):[#7;a:9]>>[#7;a:5]/[c:6](=[#7:7]\[NH;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4]):[#7;a:9]
55.6
[{"value": 48.5, "product": "O=C1C=2NC=NC2N(\\C(\\N1)=N\\NC(CCC=1OC(=NN1)C1=CC=CC=C1)=O)CCCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 55.6, "product": "O=C1C=2NC=NC2N(\\C(\\N1)=N\\NC(CCC=1OC(=NN1)C1=CC=CC=C1)=O)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
The mixture of 3-(5-phenyl-1,3,4-oxadiazol-2-yl)propanoic acid (500 mg, 20 mmol), (2E)-3-pentyl-3,7-dihydro-1H-purine-2,6-dione 2-hydrazone (480 mg, 0.0020 mol), benzotriazol-1-yloxytris(dimethylamino)phosphonium hexafluorophosphate (980 mg, 22 mmol), 4-dimethylaminopyridine (100 mg, 10 mmol), and N,N-diisopropylethyla...
10.6084/m9.figshare.5104873.v1
null
Hydrazone.Carboxylic acid
Hydrazone amide
null
null
c1nnco1.c1ccccc1.c1ncc2[nH]cnc2n1
HO-
CN(C1=CC=NC=C1)C.CN(C)C=O
null
8
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=C(O)CCc1nnc(-c2ccccc2)o1>CN(C1=CC=NC=C1)C.CN(C)C=O>CCCCCn1/c(=N/NC(=O)CCc2nnc(-c3ccccc3)o2)[nH]c(=O)c2[nH]cnc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b4ec69433a0646868f0ce761d1b9dbae
CCCCCn1/c(=N/NC(=O)CCc2nnc(-c3ccccc3)o2)[nH]c(=O)c2[nH]cnc21>>CCCCCn1c2nc[nH]c2c(=O)n2c(CCc3nnc(-c4ccccc4)o3)nnc12
O=C1C=2NC=NC2N(\C(\N1)=N\NC(CCC=1OC(=NN1)C1=CC=CC=C1)=O)CCCCC>>C(CCCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)CCC=2OC(=NN2)C2=CC=CC=C2
O=[C:15]([CH2:16][CH2:17][c:18]1[n:19][n:20][c:21](-[c:22]2[cH:23][cH:24][cH:25][cH:26][cH:27]2)[o:28]1)[NH:29]/[N:30]=[c:31]1/[n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[nH:14]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[n:14]2[...
CCCCCn1/c(=N/NC(=O)CCc2nnc(-c3ccccc3)o2)[nH]c(=O)c2[nH]cnc21
CCCCCn1c2nc[nH]c2c(=O)n2c(CCc3nnc(-c4ccccc4)o3)nnc12
null
null
C1(=CC=CC=C1)C
Aromatic Heterocycle Formation
OtherReaction
f919762557f16e8feb47c1fb62f203cd1ec4ed5f009cf276d2d0e0ec84ef6b80
78b0616e5760c6d4dadfc1fac5c58c0254d0dc7b1bf102fea4bc1349928b0776
O=c1c2[nH]cnc2[nH]c2nnc(CCc3nnc(-c4ccccc4)o3)n12
O=[C;H0;D3;+0:1](-[C:2]-[C:3])-[NH;D2;+0:4]/[N;H0;D2;+0:5]=[c;H0;D3;+0:6]1\[nH;D2;+0:7]:[c:8](=[O;D1;H0:9]):[c:10]2:[#7;a:11]:[c:12]:[#7;a:13]:[c:14]:2:[#7;a:15]:1-[C:16]>>[C:3]-[C:2]-[c;H0;D3;+0:1]1:[n;H0;D2;+0:4]:[n;H0;D2;+0:5]:[c;H0;D3;+0:6]2:[#7;a:15](-[C:16]):[c:14]3:[#7;a:13]:[c:12]:[#7;a:11]:[c:10]:3:[c:8](=[O;D...
66.7
[{"value": 66.7, "product": "C(CCCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)CCC=2OC(=NN2)C2=CC=CC=C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 66.7, "product": "C(CCCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)CCC=2OC(=NN2)C2=CC=CC=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
The mixture of N′-[(2E)-6-oxo-3-pentyl-1,3,6,7-tetrahydro-2H-purin-2-ylidene]-3-(5-phenyl-1,3,4-oxadiazol-2-yl)propanohydrazide (485 mg, 1.11 mmol) in toluene (50 mL) was heated to reflux overnight. The mixture was concentrated to yield the desired product (310 mg, 66.7%). LCMS calculated for C21H23N8O2(M+H): 419.2; fo...
10.6084/m9.figshare.5104873.v1
null
Hydrazone amide
null
c1ncc2nc[nH]c2n1
c1nc2cn3cnnc3nc2[nH]1
c1nnco1.c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
HO-
C1(=CC=CC=C1)C
null
null
CCCCCn1/c(=N/NC(=O)CCc2nnc(-c3ccccc3)o2)[nH]c(=O)c2[nH]cnc21>C1(=CC=CC=C1)C>CCCCCn1c2nc[nH]c2c(=O)n2c(CCc3nnc(-c4ccccc4)o3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-5acbf9d09b654b9cb793f0534470d859
CCCCCn1c2nc[nH]c2c(=O)n2c(CCc3nnc(-c4ccccc4)o3)nnc12.O=C1CCC(=O)N1Br>>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCc3nnc(-c4ccccc4)o3)nnc12
C(CCCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)CCC=2OC(=NN2)C2=CC=CC=C2.BrN1C(CCC1=O)=O>>BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CCC=3OC(=NN3)C3=CC=CC=C3)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([CH2:17][CH2:18][c:19]3[n:20][n:21][c:22](-[c:23]4[cH:24][cH:25][cH:26][cH:27][cH:28]4)[o:29]3)[n:30][n:31][c:32]12.O=C1CCC(=O)N1[Br:10]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:11][c:12]2[...
CCCCCn1c2nc[nH]c2c(=O)n2c(CCc3nnc(-c4ccccc4)o3)nnc12.O=C1CCC(=O)N1Br
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCc3nnc(-c4ccccc4)o3)nnc12
null
null
C1CCOC1
Functional Group Interconversion
Bromination
ec99ea20e93d70158a8c5b88a0324c2920957b29ee02a6abc4d48c347d7daa1b
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=c1c2[nH]cnc2[nH]c2nnc(CCc3nnc(-c4ccccc4)o3)n12
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[cH;D2;+0:9]:[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]>>[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[c;H0;D3;+0:9](-[Br;H0;D1;+0:1]):[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]
null
[]
70
CELSIUS
1
HOUR
The mixture of 9-pentyl-3-[2-(5-phenyl-1,3,4-oxadiazol-2-yl)ethyl]-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-5-one (53 mg, 0.13 mmol) and N-bromosuccinimide (34 mg, 0.19 mmol) in THF (20 mL) was stirred at 70° C. for 1 hour. The reaction mixture was concentrated and the residue was purified by preparative LCMS to give...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1nc2cn3cnnc3nc2[nH]1.C1CCNC1
c1nc2cn3cnnc3nc2[nH]1
c1nnco1.c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
HO-
C1CCOC1
70
1
CCCCCn1c2nc[nH]c2c(=O)n2c(CCc3nnc(-c4ccccc4)o3)nnc12.O=C1CCC(=O)N1Br>C1CCOC1>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCc3nnc(-c4ccccc4)o3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-55f0a84af50345f786b2d2064854d6f1
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=C(O)CNC(=O)OCc1ccccc1>>CCCCCn1/c(=N/NC(=O)CNC(=O)OCc2ccccc2)[nH]c(=O)c2[nH]cnc21
C(CCCC)N1/C(/NC(C=2NC=NC12)=O)=N/N.C(=O)(OCC1=CC=CC=C1)NCC(=O)O.F[P-](F)(F)(F)(F)F.N1(N=NC2=C1C=CC=C2)O[P+](N(C)C)(N(C)C)N(C)C.C(C)N(CC)CC>>O=C(CNC(OCC1=CC=CC=C1)=O)N/N=C/1\NC(C=2NC=NC2N1CCCCC)=O
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1/[c:7](=[N:8]/[NH2:9])[nH:24][c:25](=[O:26])[c:27]2[nH:28][cH:29][n:30][c:31]12.O[C:10](=[O:11])[CH2:12][NH:13][C:14](=[O:15])[O:16][CH2:17][c:18]1[cH:19][cH:20][cH:21][cH:22][cH:23]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1/[c:7](=[N:8]/[NH:9][C:10](=[O:11])[CH2:12][NH:13][C:...
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=C(O)CNC(=O)OCc1ccccc1
CCCCCn1/c(=N/NC(=O)CNC(=O)OCc2ccccc2)[nH]c(=O)c2[nH]cnc21
null
null
CN(C)C=O.CCOC(=O)C
Acylation
Carboxylic acid with primary amine to amide
e50d935ef072f0718d4e131af3df793f26e2f0a63884801973739584ab6e55ba
2740512737e2508c1c8d407d0ee271fd1e1c46ad16223e8e2fc1e12936af0dea
O=C(CNC(=O)OCc1ccccc1)N/N=c1\[nH]c(=O)c2[nH]cnc2[nH]1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#7:4]-[C:5]=[O;D1;H0:6].[#7;a:7]/[c:8](=[#7:9]\[NH2;D1;+0:10]):[#7;a:11]>>[#7;a:7]/[c:8](=[#7:9]\[NH;D2;+0:10]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[#7:4]-[C:5]=[O;D1;H0:6]):[#7;a:11]
144.8
[{"value": 86.0, "product": "O=C(CNC(OCC1=CC=CC=C1)=O)N/N=C/1\\NC(C=2NC=NC2N1CCCCC)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 144.8, "product": "O=C(CNC(OCC1=CC=CC=C1)=O)N/N=C/1\\NC(C=2NC=NC2N1CCCCC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
The mixture of (2E)-3-pentyl-3,7-dihydro-1H-purine-2,6-dione 2-hydrazone (0.50 g, 0.0021 mol), N-carbobenzyloxyglycine (0.49 g, 0.0023 mol), benzotriazol-1-yloxytris(dimethylamino)phosphonium hexafluorophosphate (1.0 g, 2.3 mmol) and triethylamine (0.59 mL, 0.0042 mol) in DMF (20 mL) was stirred at room temperature ove...
10.6084/m9.figshare.5104873.v1
null
Hydrazone.Carboxylic acid
Hydrazone amide
null
null
c1ccccc1.c1ncc2[nH]cnc2n1
HO-
CN(C)C=O.CCOC(=O)C
null
8
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=C(O)CNC(=O)OCc1ccccc1>CN(C)C=O.CCOC(=O)C>CCCCCn1/c(=N/NC(=O)CNC(=O)OCc2ccccc2)[nH]c(=O)c2[nH]cnc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-2773aaf43dfa4286919f9a00d95706a5
CCCCCn1/c(=N/NC(=O)CNC(=O)OCc2ccccc2)[nH]c(=O)c2[nH]cnc21>>CCCCCn1c2nc[nH]c2c(=O)n2c(CNC(=O)OCc3ccccc3)nnc12
O=C(CNC(OCC1=CC=CC=C1)=O)N/N=C/1\NC(C=2NC=NC2N1CCCCC)=O>>O=C1C=2NC=NC2N(C=2N1C(=NN2)CNC(OCC2=CC=CC=C2)=O)CCCCC
O=[C:15]([CH2:16][NH:17][C:18](=[O:19])[O:20][CH2:21][c:22]1[cH:23][cH:24][cH:25][cH:26][cH:27]1)[NH:28]/[N:29]=[c:30]1/[n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[nH:14]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[n:14]2[c:15]([...
CCCCCn1/c(=N/NC(=O)CNC(=O)OCc2ccccc2)[nH]c(=O)c2[nH]cnc21
CCCCCn1c2nc[nH]c2c(=O)n2c(CNC(=O)OCc3ccccc3)nnc12
null
null
C1(=CC=CC=C1)C
Aromatic Heterocycle Formation
OtherReaction
f919762557f16e8feb47c1fb62f203cd1ec4ed5f009cf276d2d0e0ec84ef6b80
78b0616e5760c6d4dadfc1fac5c58c0254d0dc7b1bf102fea4bc1349928b0776
O=C(NCc1nnc2[nH]c3nc[nH]c3c(=O)n12)OCc1ccccc1
O=[C;H0;D3;+0:1](-[C:2]-[#7:3]-[C:4]=[O;D1;H0:5])-[NH;D2;+0:6]/[N;H0;D2;+0:7]=[c;H0;D3;+0:8]1\[nH;D2;+0:9]:[c:10](=[O;D1;H0:11]):[c:12]2:[#7;a:13]:[c:14]:[#7;a:15]:[c:16]:2:[#7;a:17]:1-[C:18]>>[C:18]-[#7;a:17]1:[c:16]2:[#7;a:15]:[c:14]:[#7;a:13]:[c:12]:2:[c:10](=[O;D1;H0:11]):[n;H0;D3;+0:9]2:[c;H0;D3;+0:1](-[C:2]-[#7:3...
87.2
[{"value": 87.0, "product": "O=C1C=2NC=NC2N(C=2N1C(=NN2)CNC(OCC2=CC=CC=C2)=O)CCCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 87.2, "product": "O=C1C=2NC=NC2N(C=2N1C(=NN2)CNC(OCC2=CC=CC=C2)=O)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
The solution of benzyl 2-oxo-2-[(2E)-2-(6-oxo-3-pentyl-1,3,6,7-tetrahydro-2H-purin-2-ylidene)hydrazino]ethylcarbamate (0.60 g, 0.84 mmol) in toluene (30 mL) was refluxed overnight. M+H=410.1. The product was precipitated from the reaction mixture and filtered to give the desired product (300 mg, 87%). LCMS calculated f...
10.6084/m9.figshare.5104873.v1
null
Hydrazone amide
null
c1ncc2nc[nH]c2n1
c1nc2cn3cnnc3nc2[nH]1
c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
HO-
C1(=CC=CC=C1)C
null
null
CCCCCn1/c(=N/NC(=O)CNC(=O)OCc2ccccc2)[nH]c(=O)c2[nH]cnc21>C1(=CC=CC=C1)C>CCCCCn1c2nc[nH]c2c(=O)n2c(CNC(=O)OCc3ccccc3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-509439a3ab9a4aa4a6828bf58a381a1e
CCCCCn1c2nc[nH]c2c(=O)n2c(CNC(=O)OCc3ccccc3)nnc12>>CCCCCn1c2nc[nH]c2c(=O)n2c(CN)nnc12
O=C1C=2NC=NC2N(C=2N1C(=NN2)CNC(OCC2=CC=CC=C2)=O)CCCCC.Cl>>Cl.NCC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O
O=C(OCc1ccccc1)[NH:17][CH2:16][c:15]1[n:14]2[c:12](=[O:13])[c:11]3[c:7]([n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:20]2[n:19][n:18]1)[n:8][cH:9][nH:10]3>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[n:14]2[c:15]([CH2:16][NH2:17])[n:18][n:19][c:20]12
CCCCCn1c2nc[nH]c2c(=O)n2c(CNC(=O)OCc3ccccc3)nnc12
CCCCCn1c2nc[nH]c2c(=O)n2c(CN)nnc12
null
[Pd]
CO
Reduction
Hydrogenolysis of amides/imides/carbamates
087b6600ba91d3df931fe6979f2445c192cbfd59e04fd2d8a10f7c7573ac669f
4e549866ec1acadec4c84aaf8495992a28ec78d8ea5ef1b9f44dd843b0dcb7d4
O=c1c2[nH]cnc2[nH]c2nncn12
O=C(-O-C-c1:c:c:c:c:c:1)-[NH;D2;+0:1]-[C:2]-[c:3](:[#7;a:4]):[#7;a:5]:[#7;a:6]>>[#7;a:4]:[c:3](-[C:2]-[NH2;D1;+0:1]):[#7;a:5]:[#7;a:6]
92
[{"value": 92.0, "product": "Cl.NCC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
To the solution of benzyl [(5-oxo-9-pentyl-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-3-yl)methyl]carbamate (0.30 g, 0.73 mmol) in methanol (20 mL) and 1 mL of conc. HCl was added 110% Pd/C under N2. The mixture was shaken under 30 PSI H2 for 3 hours. The reaction mixture was filtered through celite and concentrated to...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether
Primary amine
c1ccccc1
null
c1nc2cn3cnnc3nc2[nH]1
HO-
[Pd].CO
null
3
CCCCCn1c2nc[nH]c2c(=O)n2c(CNC(=O)OCc3ccccc3)nnc12>[Pd].CO>CCCCCn1c2nc[nH]c2c(=O)n2c(CN)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-88222f041af54668a0322272cf79d9b1
CCCCCn1c2nc[nH]c2c(=O)n2c(CN)nnc12.O=C(O)c1ccccc1>>CCCCCn1c2nc[nH]c2c(=O)n2c(CNC(=O)c3ccccc3)nnc12
Cl.NCC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O.C(C1=CC=CC=C1)(=O)O.F[P-](F)(F)(F)(F)F.N1(N=NC2=C1C=CC=C2)O[P+](N(C)C)(N(C)C)N(C)C.C(C)N(CC)CC>>O=C1C=2NC=NC2N(C=2N1C(=NN2)CNC(C2=CC=CC=C2)=O)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[n:14]2[c:15]([CH2:16][NH2:17])[n:26][n:27][c:28]12.O[C:18](=[O:19])[c:20]1[cH:21][cH:22][cH:23][cH:24][cH:25]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[n:14]2[c:15]([CH2:16][NH:17][C:1...
CCCCCn1c2nc[nH]c2c(=O)n2c(CN)nnc12.O=C(O)c1ccccc1
CCCCCn1c2nc[nH]c2c(=O)n2c(CNC(=O)c3ccccc3)nnc12
null
null
CN(C)C=O
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(NCc1nnc2[nH]c3nc[nH]c3c(=O)n12)c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[#7;a:6]:[c:7](-[C:8]-[NH2;D1;+0:9]):[#7;a:10]:[#7;a:11]>>[#7;a:6]:[c:7](-[C:8]-[NH;D2;+0:9]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]):[#7;a:10]:[#7;a:11]
77.5
[{"value": 77.0, "product": "O=C1C=2NC=NC2N(C=2N1C(=NN2)CNC(C2=CC=CC=C2)=O)CCCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 77.5, "product": "O=C1C=2NC=NC2N(C=2N1C(=NN2)CNC(C2=CC=CC=C2)=O)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
The mixture of 3-(aminomethyl)-9-pentyl-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-5-one hydrochloride (160 mg, 0.51 mmol), [B] benzoic Acid (0.069 g, 0.56 mmol), benzotriazol-1-yloxytris(dimethylamino)phosphonium hexafluorophosphate (0.25 g, 0.56 mmol) and triethylamine (0.21 mL, 1.5 mmol) in DMF (10 mL) was stirred a...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
HO-
CN(C)C=O
null
8
CCCCCn1c2nc[nH]c2c(=O)n2c(CN)nnc12.O=C(O)c1ccccc1>CN(C)C=O>CCCCCn1c2nc[nH]c2c(=O)n2c(CNC(=O)c3ccccc3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-b8a4e123163446e8907c9d8ce735263f
CCCCCn1c2nc[nH]c2c(=O)n2c(CNC(=O)c3ccccc3)nnc12.O=C1CCC(=O)N1Br>>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CNC(=O)c3ccccc3)nnc12
O=C1C=2NC=NC2N(C=2N1C(=NN2)CNC(C2=CC=CC=C2)=O)CCCCC.BrN1C(CCC1=O)=O>>BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CNC(C3=CC=CC=C3)=O)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([CH2:17][NH:18][C:19](=[O:20])[c:21]3[cH:22][cH:23][cH:24][cH:25][cH:26]3)[n:27][n:28][c:29]12.O=C1CCC(=O)N1[Br:10]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:11][c:12]2[c:13](=[O:14])[n:15]2...
CCCCCn1c2nc[nH]c2c(=O)n2c(CNC(=O)c3ccccc3)nnc12.O=C1CCC(=O)N1Br
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CNC(=O)c3ccccc3)nnc12
null
null
C1CCOC1
Functional Group Interconversion
Bromination
ec99ea20e93d70158a8c5b88a0324c2920957b29ee02a6abc4d48c347d7daa1b
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=C(NCc1nnc2[nH]c3nc[nH]c3c(=O)n12)c1ccccc1
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[cH;D2;+0:9]:[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]>>[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[c;H0;D3;+0:9](-[Br;H0;D1;+0:1]):[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]
null
[]
70
CELSIUS
1
HOUR
To the solution of N-[(5-oxo-9-pentyl-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-3-yl)methyl]benzamide (0.11 g, 0.28 mmol) in THF (10 mL) was added N-Bromosuccinimide (0.076 g, 0.42 mmol). The mixture was stirred at 70° C. for 1 hour. The reaction mixture was concentrated and purified by preparative LCMS. LCMS calculat...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1nc2cn3cnnc3nc2[nH]1.C1CCNC1
c1nc2cn3cnnc3nc2[nH]1
c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
HO-
C1CCOC1
70
1
CCCCCn1c2nc[nH]c2c(=O)n2c(CNC(=O)c3ccccc3)nnc12.O=C1CCC(=O)N1Br>C1CCOC1>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CNC(=O)c3ccccc3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-87c293b71b634136b711cbd10d1cee34
CCCCCn1c(=S)[nH]c(=O)c2[nH]cnc21.COS(=O)(=O)OC>>CCCCCn1c(SC)nc(=O)c2[nH]cnc21
C(CCCC)N1C(NC(C=2NC=NC12)=O)=S.S(=O)(=O)(OC)OC.C(C)(=O)O>>CSC1=NC(C=2NC=NC2N1CCCCC)=O
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7](=[S:8])[nH:10][c:11](=[O:12])[c:13]2[nH:14][cH:15][n:16][c:17]12.COS(=O)(=O)O[CH3:9]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]([S:8][CH3:9])[n:10][c:11](=[O:12])[c:13]2[nH:14][cH:15][n:16][c:17]12
CCCCCn1c(=S)[nH]c(=O)c2[nH]cnc21.COS(=O)(=O)OC
CCCCCn1c(SC)nc(=O)c2[nH]cnc21
null
null
O.[OH-].[Na+]
Heteroatom Alkylation and Arylation
OtherReaction
0161fed9f1388ec369b7cbafe281cc52a2e7ee362447238b9354e3768807eefa
e73b6e23c9de2770653dfe1c031448ae08eae1a1e8b31e289bfc4b4719e52064
O=c1nc[nH]c2nc[nH]c12
C-O-S(=O)(=O)-O-[CH3;D1;+0:1].[C:2]-[#7;a:3]1:[c:4]2:[#7;a:5]:[c:6]:[#7;a:7]:[c:8]:2:[c:9](=[O;D1;H0:10]):[nH;D2;+0:11]:[c;H0;D3;+0:12]:1=[S;H0;D1;+0:13]>>[C:2]-[#7;a:3]1:[c:4]2:[#7;a:5]:[c:6]:[#7;a:7]:[c:8]:2:[c:9](=[O;D1;H0:10]):[n;H0;D2;+0:11]:[c;H0;D3;+0:12]:1-[S;H0;D2;+0:13]-[CH3;D1;+0:1]
40
[{"value": 40.0, "product": "CSC1=NC(C=2NC=NC2N1CCCCC)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 39.9, "product": "CSC1=NC(C=2NC=NC2N1CCCCC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a solution of 3-pentyl-2-thioxo-1,2,3,7-tetrahydro-6H-purin-6-one (13.0 g, 54.6 mmol) in 2 M of sodium hydroxide in water (250 mL) was added dimethyl sulfate (6.2 mL, 66 mmol), and the reaction mixture was stirred at room temperature for 1 hour, then neutralized with acetic acid. The precipitate was collected by fil...
10.6084/m9.figshare.5104873.v1
null
Thiocarbonyl
Monosulfide
c1ncc2[nH]cnc2n1
c1ncc2[nH]cnc2n1
c1ncc2[nH]cnc2n1
HO-
O.[OH-].[Na+]
null
1
CCCCCn1c(=S)[nH]c(=O)c2[nH]cnc21.COS(=O)(=O)OC>O.[OH-].[Na+]>CCCCCn1c(SC)nc(=O)c2[nH]cnc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-58cc3e97c2ca4db5a597f0230a3f3407
CCCCCn1c(SC)nc(=O)c2[nH]cnc21.N>>CCCCCn1c(N)nc(=O)c2[nH]cnc21
CSC1=NC(C=2NC=NC2N1CCCCC)=O.[OH-].N>>NC1=NC(C=2NC=NC2N1CCCCC)=O
CS[c:7]1[n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:16]2[c:12]([c:10](=[O:11])[n:9]1)[nH:13][cH:14][n:15]2.[NH3:8]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]([NH2:8])[n:9][c:10](=[O:11])[c:12]2[nH:13][cH:14][n:15][c:16]12
CCCCCn1c(SC)nc(=O)c2[nH]cnc21.N
CCCCCn1c(N)nc(=O)c2[nH]cnc21
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
f500e8e89d97d64d15e1420f37f84c3739bb246c9e00620675f4ee3b3fc90072
fe235a2b93109096a39cf211c5494ce5db3b96d4e6b4b4ac937f939eb8bec4c8
O=c1nc[nH]c2nc[nH]c12
C-S-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4](:[#7;a:5]):[c:6](:[#7;a:7]):[#7;a:8]:1-[C:9].[NH3;D0;+0:10]>>[#7;a:5]:[c:4]1:[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[NH2;D1;+0:10]):[#7;a:8](-[C:9]):[c:6]:1:[#7;a:7]
68
[{"value": 68.0, "product": "NC1=NC(C=2NC=NC2N1CCCCC)=O", "details": "PERCENTYIELD", "is_desired": false}]
100
CELSIUS
4
DAY
2-(Methylthio)-3-pentyl-3,7-dihydro-6H-purin-6-one (5.0 g, 0.020 mol) was mixed with 100 ml of 28% ammonia hydroxide in a seal tube. The mixture was stirred at 100° C. for 4 days. After cooling to room temperature, the solid was filtered and dried to yield the desired product (3.0 g, 68%). LCMS calculated for C10H16N5O...
10.6084/m9.figshare.5104873.v1
null
Monosulfide
Primary amine
c1ncc2[nH]cnc2n1
c1ncc2[nH]cnc2n1
c1ncc2[nH]cnc2n1
Other
null
100
96
CCCCCn1c(SC)nc(=O)c2[nH]cnc21.N>>CCCCCn1c(N)nc(=O)c2[nH]cnc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-7b254ddca196496dbc382f1be0f01e0c
CCCCCn1c(=N)[nH]c(=O)c2[nH]cnc21.NN>>CCCCCn1c(=N)n(N)c(=O)c2[nH]cnc21
N=C1NC(C=2NC=NC2N1CCCCC)=O.NN>>NN1C(N(C=2N=CNC2C1=O)CCCCC)=N
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7](=[NH:8])[nH:9][c:11](=[O:12])[c:13]2[nH:14][cH:15][n:16][c:17]12.N[NH2:10]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7](=[NH:8])[n:9]([NH2:10])[c:11](=[O:12])[c:13]2[nH:14][cH:15][n:16][c:17]12
CCCCCn1c(=N)[nH]c(=O)c2[nH]cnc21.NN
CCCCCn1c(=N)n(N)c(=O)c2[nH]cnc21
null
null
O
Miscellaneous
OtherReaction
0f4a18c44e3db037bff63652b6a4d971a509f3c51b7e12e9057738e30dfedc4d
ae87b85154e4ed9f19e174b708d1b263c1808f04035e196936e83905c9eea0fd
N=c1[nH]c(=O)c2[nH]cnc2[nH]1
N-[NH2;D1;+0:1].[C:2]-[#7;a:3]1:[c:4]2:[#7;a:5]:[c:6]:[#7;a:7]:[c:8]:2:[c:9](=[O;D1;H0:10]):[nH;D2;+0:11]:[c:12]:1=[N;D1;H1:13]>>[C:2]-[#7;a:3]1:[c:4]2:[#7;a:5]:[c:6]:[#7;a:7]:[c:8]:2:[c:9](=[O;D1;H0:10]):[n;H0;D3;+0:11](-[NH2;D1;+0:1]):[c:12]:1=[N;D1;H1:13]
null
[]
null
null
null
null
A solution of 2-imino-3-pentyl-1,2,3,7-tetrahydro-6h-purin-6-one (750 mg, 3.39 mmol) and 18 m of hydrazine in water (30 ml) was stirred at 150° C. for 30 min on a microwave reactor. The reaction was diluted with water and extracted with ethyl acetate three times, dried with sodium sulfate, filtered, and concentrated in...
10.6084/m9.figshare.5104873.v1
null
Hydrazine
Primary amine
c1ncc2[nH]cnc2n1
c1ncc2[nH]cnc2n1
c1ncc2[nH]cnc2n1
Other
O
null
null
CCCCCn1c(=N)[nH]c(=O)c2[nH]cnc21.NN>O>CCCCCn1c(=N)n(N)c(=O)c2[nH]cnc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-746a3899625e484b9b62674d97b7a641
CCCCCn1c(=N)n(N)c(=O)c2[nH]cnc21>>CCCCCn1c2nc[nH]c2c(=O)n2ncnc12
NN1C(N(C=2N=CNC2C1=O)CCCCC)=N.C(OCC)([O-])[O-]>>C(CCCC)N1C=2N(C(C=3NC=NC13)=O)N=CN2
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[n:14]([NH2:15])[c:18]1=[NH:17]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[n:14]2[n:15][cH:16][n:17][c:18]12
CCCCCn1c(=N)n(N)c(=O)c2[nH]cnc21
CCCCCn1c2nc[nH]c2c(=O)n2ncnc12
null
null
null
Aromatic Heterocycle Formation
OtherReaction
42583e3aaec0e678b7fe424f1573058d717f460b288147923b1c6f65cb69b8ec
0c2e6cfe0bdb8f8cd78303a7637b3ef339f807f5bc27c4a22ad516ce20b37476
O=c1c2[nH]cnc2[nH]c2ncnn12
[#7;a:1]:[c:2]1:[c:3]:[#7;a:4](-[NH2;D1;+0:5]):[c;H0;D3;+0:6](=[NH;D1;+0:7]):[#7;a:8](-[C:9]):[c:10]:1:[#7;a:11]>>[#7;a:1]:[c:2]1:[c:3]:[#7;a:4]2:[n;H0;D2;+0:5]:[c:12]:[n;H0;D2;+0:7]:[c;H0;D3;+0:6]:2:[#7;a:8](-[C:9]):[c:10]:1:[#7;a:11]
20.3
[{"value": 20.0, "product": "C(CCCC)N1C=2N(C(C=3NC=NC13)=O)N=CN2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 20.3, "product": "C(CCCC)N1C=2N(C(C=3NC=NC13)=O)N=CN2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
6
HOUR
The mixture of 1-amino-2-imino-3-pentyl-1,2,3,7-tetrahydro-6H-purin-6-one (0.10 g, 0.4 mmol) and ethyl orthoformate (5 mL, 30 mmol) was stirred at 100° C. for 6 hours. The reaction mixture was concentrated and purified by preparative LCMS to yield the desired product (20 mg, 20%). LCMS calculated for C11H15N6O(M+H): 24...
10.6084/m9.figshare.5104873.v1
null
Primary amine
null
c1ncc2nc[nH]c2n1
c1nc2nc3[nH]cnc3cn2n1
c1nc2nc3[nH]cnc3cn2n1
Other
null
100
6
CCCCCn1c(=N)n(N)c(=O)c2[nH]cnc21>>CCCCCn1c2nc[nH]c2c(=O)n2ncnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-cd5a6e849daf43f79ba7675cb3f849d4
CCCCCn1c2nc[nH]c2c(=O)n2ncnc12.O=C1CCC(=O)N1Br>>CCCCCn1c2nc(Br)[nH]c2c(=O)n2ncnc12
C(CCCC)N1C=2N(C(C=3NC=NC13)=O)N=CN2.BrN1C(CCC1=O)=O>>BrC1=NC=2N(C=3N(C(C2N1)=O)N=CN3)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:11][c:12]2[c:13](=[O:14])[n:15]2[n:16][cH:17][n:18][c:19]12.O=C1CCC(=O)N1[Br:10]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:11][c:12]2[c:13](=[O:14])[n:15]2[n:16][cH:17][n:18][c:19]12
CCCCCn1c2nc[nH]c2c(=O)n2ncnc12.O=C1CCC(=O)N1Br
CCCCCn1c2nc(Br)[nH]c2c(=O)n2ncnc12
null
null
O1CCCC1
Functional Group Interconversion
Bromination
e711ed5c7fb7355144c6c6d25a210978a28c6ca3b2370bedf2b4f5d98ce282dc
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=c1c2[nH]cnc2[nH]c2ncnn12
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#7;a:2]:[#7;a:3]1:[c:4]:[c:5]2:[#7;a:6]:[cH;D2;+0:7]:[#7;a:8]:[c:9]:2:[#7;a:10](-[C:11]):[c:12]:1:[#7;a:13]>>[#7;a:2]:[#7;a:3]1:[c:4]:[c:5]2:[#7;a:6]:[c;H0;D3;+0:7](-[Br;H0;D1;+0:1]):[#7;a:8]:[c:9]:2:[#7;a:10](-[C:11]):[c:12]:1:[#7;a:13]
12.4
[{"value": 12.4, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)N=CN3)CCCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 12.4, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)N=CN3)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
70
CELSIUS
1
HOUR
To the mixture of 4-pentyl-1,4-dihydro-9H-[1,2,4]triazolo[1,5-a]purin-9-one (19 mg, 0.077 mmol) in tetrahydrofuran (10 mL) was added N-bromosuccinimide (20 mg, 0.12 mol) at rt. The mixture was stirred at 70° C. for 1 hour. The mixture was concentrated and purified by preparative LCMS to yield the desired product (3.10 ...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1nc2nc3[nH]cnc3cn2n1.C1CCNC1
c1nc2nc3[nH]cnc3cn2n1
c1nc2nc3[nH]cnc3cn2n1
HO-
O1CCCC1
70
1
CCCCCn1c2nc[nH]c2c(=O)n2ncnc12.O=C1CCC(=O)N1Br>O1CCCC1>CCCCCn1c2nc(Br)[nH]c2c(=O)n2ncnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ec329f6c78014479a2009b41f7037f75
COC(=O)CC(C)c1nc(-c2ccccc2)no1>>O=C(O)CCCc1nc(-c2ccccc2)no1
Cl.C1(=CC=CC=C1)C1=NOC(=N1)C(CC(=O)OC)C.[OH-].[Na+].CO>>C1(=CC=CC=C1)C1=NOC(=N1)CCCC(=O)O
C[O:3][C:2](=[O:1])[CH2:4][CH:6]([CH3:5])[c:7]1[n:8][c:9](-[c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[n:16][o:17]1>>[O:1]=[C:2]([OH:3])[CH2:4][CH2:5][CH2:6][c:7]1[n:8][c:9](-[c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[n:16][o:17]1
COC(=O)CC(C)c1nc(-c2ccccc2)no1
O=C(O)CCCc1nc(-c2ccccc2)no1
null
null
null
Miscellaneous
OtherReaction
16eb0e22715fadede32e44259800ac2375ae7dbc609f9ec677d59917bae07bec
b51da43dbb7140dac708518f8dbf83c5b067214819134afdb3f427285d08d6f8
c1ccc(-c2ncon2)cc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[CH2;D2;+0:4]-[CH;D3;+0:5](-[CH3;D1;+0:6])-[c:7]1:[#7;a:8]:[c:9]:[#7;a:10]:[#8;a:11]:1>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[CH2;D2;+0:4]-[CH2;D2;+0:6]-[CH2;D2;+0:5]-[c:7]1:[#7;a:8]:[c:9]:[#7;a:10]:[#8;a:11]:1
99
[{"value": 99.0, "product": "C1(=CC=CC=C1)C1=NOC(=N1)CCCC(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
To a solution of methyl 3-(3-phenyl-1,2,4-oxadiazol-5-yl)butanoate (1.53 g, 6.21 mmole) in methanol (10 ml) was added 1N NaOH (10 mL). After stirring at room temperature for 2 hours, the reaction solution was acidified to pH=3-4 with 6N HCl under an ice bath and then extracted with ethyl acetate three times. The combin...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ncon1.c1ccccc1
Other
null
null
2
COC(=O)CC(C)c1nc(-c2ccccc2)no1>>O=C(O)CCCc1nc(-c2ccccc2)no1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-edc1fd367db644c7aaa6b540b0558972
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=C(O)CCCc1nc(-c2ccccc2)no1>>CCCCCn1/c(=N/NC(=O)CCCc2nc(-c3ccccc3)no2)[nH]c(=O)c2[nH]cnc21
C1(=CC=CC=C1)C1=NOC(=N1)CCCC(=O)O.C(CCCC)N1/C(/NC(C=2NC=NC12)=O)=N/N.F[P-](F)(F)(F)(F)F.N1(N=NC2=C1C=CC=C2)O[P+](N(C)C)(N(C)C)N(C)C.C(C)N(CC)CC>>O=C1C=2NC=NC2N(\C(\N1)=N\NC(CCCC1=NC(=NO1)C1=CC=CC=C1)=O)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1/[c:7](=[N:8]/[NH2:9])[nH:26][c:27](=[O:28])[c:29]2[nH:30][cH:31][n:32][c:33]12.O[C:10](=[O:11])[CH2:12][CH2:13][CH2:14][c:15]1[n:16][c:17](-[c:18]2[cH:19][cH:20][cH:21][cH:22][cH:23]2)[n:24][o:25]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1/[c:7](=[N:8]/[NH:9][C:10](=[O:11])[CH...
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=C(O)CCCc1nc(-c2ccccc2)no1
CCCCCn1/c(=N/NC(=O)CCCc2nc(-c3ccccc3)no2)[nH]c(=O)c2[nH]cnc21
null
null
O.CN(C)C=O
Acylation
Carboxylic acid with primary amine to amide
e50d935ef072f0718d4e131af3df793f26e2f0a63884801973739584ab6e55ba
2740512737e2508c1c8d407d0ee271fd1e1c46ad16223e8e2fc1e12936af0dea
O=C(CCCc1nc(-c2ccccc2)no1)N/N=c1\[nH]c(=O)c2[nH]cnc2[nH]1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4].[#7;a:5]/[c:6](=[#7:7]\[NH2;D1;+0:8]):[#7;a:9]>>[#7;a:5]/[c:6](=[#7:7]\[NH;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4]):[#7;a:9]
99.5
[{"value": 99.0, "product": "O=C1C=2NC=NC2N(\\C(\\N1)=N\\NC(CCCC1=NC(=NO1)C1=CC=CC=C1)=O)CCCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 99.5, "product": "O=C1C=2NC=NC2N(\\C(\\N1)=N\\NC(CCCC1=NC(=NO1)C1=CC=CC=C1)=O)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
A mixture of 4-(3-phenyl-1,2,4-oxadiazol-5-yl)butanoic acid (1.44 g, 6.20 mmol), (2e)-3-pentyl-3,7-dihydro-1h-purine-2,6-dione 2-hydrazone (1.61 g, 6.82 mmol), benzotriazol-1-yloxytris(dimethylamino)phosphonium hexafluorophosphate (3.02 g, 6.82 mmol) and triethylamine (1.73 ml, 12.4 mmol) in DMF (30 ml) was stirred at ...
10.6084/m9.figshare.5104873.v1
null
Hydrazone.Carboxylic acid
Hydrazone amide
null
null
c1ncon1.c1ccccc1.c1ncc2[nH]cnc2n1
HO-
O.CN(C)C=O
null
8
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=C(O)CCCc1nc(-c2ccccc2)no1>O.CN(C)C=O>CCCCCn1/c(=N/NC(=O)CCCc2nc(-c3ccccc3)no2)[nH]c(=O)c2[nH]cnc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-104fb25fc2a046589e3c6ef947115662
CCCCCn1/c(=N/NC(=O)CCCc2nc(-c3ccccc3)no2)[nH]c(=O)c2[nH]cnc21>>CCCCCn1c2nc[nH]c2c(=O)n2c(CCCc3nc(-c4ccccc4)no3)nnc12
O=C1C=2NC=NC2N(\C(\N1)=N\NC(CCCC1=NC(=NO1)C1=CC=CC=C1)=O)CCCCC>>C(CCCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)CCCC2=NC(=NO2)C2=CC=CC=C2
O=[C:15]([CH2:16][CH2:17][CH2:18][c:19]1[n:20][c:21](-[c:22]2[cH:23][cH:24][cH:25][cH:26][cH:27]2)[n:28][o:29]1)[NH:30]/[N:31]=[c:32]1/[n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[nH:14]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])...
CCCCCn1/c(=N/NC(=O)CCCc2nc(-c3ccccc3)no2)[nH]c(=O)c2[nH]cnc21
CCCCCn1c2nc[nH]c2c(=O)n2c(CCCc3nc(-c4ccccc4)no3)nnc12
null
null
C1(=CC=CC=C1)C
Aromatic Heterocycle Formation
OtherReaction
f919762557f16e8feb47c1fb62f203cd1ec4ed5f009cf276d2d0e0ec84ef6b80
78b0616e5760c6d4dadfc1fac5c58c0254d0dc7b1bf102fea4bc1349928b0776
O=c1c2[nH]cnc2[nH]c2nnc(CCCc3nc(-c4ccccc4)no3)n12
O=[C;H0;D3;+0:1](-[C:2]-[C:3])-[NH;D2;+0:4]/[N;H0;D2;+0:5]=[c;H0;D3;+0:6]1\[nH;D2;+0:7]:[c:8](=[O;D1;H0:9]):[c:10]2:[#7;a:11]:[c:12]:[#7;a:13]:[c:14]:2:[#7;a:15]:1-[C:16]>>[C:3]-[C:2]-[c;H0;D3;+0:1]1:[n;H0;D2;+0:4]:[n;H0;D2;+0:5]:[c;H0;D3;+0:6]2:[#7;a:15](-[C:16]):[c:14]3:[#7;a:13]:[c:12]:[#7;a:11]:[c:10]:3:[c:8](=[O;D...
74
[{"value": 74.0, "product": "C(CCCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)CCCC2=NC(=NO2)C2=CC=CC=C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 73.8, "product": "C(CCCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)CCCC2=NC(=NO2)C2=CC=CC=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
The mixture of N′-[(2E)-6-oxo-3-pentyl-1,3,6,7-tetrahydro-2H-purin-2-ylidene]-4-(3-phenyl-1,2,4-oxadiazol-5-yl)butanohydrazide (2.78 g, 6.17 mmol) in toluene (100 ml) was refluxed for 2 hours. After cooling to room temperature, the solid was filtered, washed with ethyl acetate/Hexane (1:9) and dried to give the desired...
10.6084/m9.figshare.5104873.v1
null
Hydrazone amide
null
c1ncc2nc[nH]c2n1
c1nc2cn3cnnc3nc2[nH]1
c1ncon1.c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
HO-
C1(=CC=CC=C1)C
null
null
CCCCCn1/c(=N/NC(=O)CCCc2nc(-c3ccccc3)no2)[nH]c(=O)c2[nH]cnc21>C1(=CC=CC=C1)C>CCCCCn1c2nc[nH]c2c(=O)n2c(CCCc3nc(-c4ccccc4)no3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-118a8b47000742aebe0f51e7ea0e8e80
CCCCCn1c2nc[nH]c2c(=O)n2c(CCCc3nc(-c4ccccc4)no3)nnc12.O=C1CCC(=O)N1Br>>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCCc3nc(-c4ccccc4)no3)nnc12
C(CCCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)CCCC2=NC(=NO2)C2=CC=CC=C2.BrN1C(CCC1=O)=O>>BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CCCC3=NC(=NO3)C3=CC=CC=C3)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([CH2:17][CH2:18][CH2:19][c:20]3[n:21][c:22](-[c:23]4[cH:24][cH:25][cH:26][cH:27][cH:28]4)[n:29][o:30]3)[n:31][n:32][c:33]12.O=C1CCC(=O)N1[Br:10]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:11]...
CCCCCn1c2nc[nH]c2c(=O)n2c(CCCc3nc(-c4ccccc4)no3)nnc12.O=C1CCC(=O)N1Br
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCCc3nc(-c4ccccc4)no3)nnc12
null
null
C1CCOC1
Functional Group Interconversion
Bromination
ec99ea20e93d70158a8c5b88a0324c2920957b29ee02a6abc4d48c347d7daa1b
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=c1c2[nH]cnc2[nH]c2nnc(CCCc3nc(-c4ccccc4)no3)n12
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[cH;D2;+0:9]:[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]>>[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[c;H0;D3;+0:9](-[Br;H0;D1;+0:1]):[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]
21
[{"value": 21.0, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CCCC3=NC(=NO3)C3=CC=CC=C3)CCCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 20.6, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CCCC3=NC(=NO3)C3=CC=CC=C3)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
70
CELSIUS
1
HOUR
To the solution of 9-pentyl-3-[3-(3-phenyl-1,2,4-oxadiazol-5-yl)propyl]-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-5-one (0.50 g, 1.16 mmole) in THF (125 ml) at room temperature was added N-bromosuccinimide (0.309 g, 1.73 mmole). The mixture was stirred at 70° C. for 1 h. The mixture was concentrated and purified by pr...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1nc2cn3cnnc3nc2[nH]1.C1CCNC1
c1nc2cn3cnnc3nc2[nH]1
c1ncon1.c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
HO-
C1CCOC1
70
1
CCCCCn1c2nc[nH]c2c(=O)n2c(CCCc3nc(-c4ccccc4)no3)nnc12.O=C1CCC(=O)N1Br>C1CCOC1>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCCc3nc(-c4ccccc4)no3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-183ec978cfe24da39389a33fc446e25c
CCOC(=O)CCCBr.c1ccc(-c2cn[nH]c2)cc1>>CCOC(=O)CCCn1cc(-c2ccccc2)cn1
BrCCCC(=O)OCC.C1(=CC=CC=C1)C=1C=NNC1.C(=O)([O-])[O-].[K+].[K+]>>C1(=CC=CC=C1)C=1C=NN(C1)CCCC(=O)OCC
Br[CH2:8][CH2:7][CH2:6][C:4]([O:3][CH2:2][CH3:1])=[O:5].[nH:9]1[cH:10][c:11](-[c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[cH:18][n:19]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][CH2:7][CH2:8][n:9]1[cH:10][c:11](-[c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[cH:18][n:19]1
CCOC(=O)CCCBr.c1ccc(-c2cn[nH]c2)cc1
CCOC(=O)CCCn1cc(-c2ccccc2)cn1
null
null
O.CN(C)C=O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
31849359320dc3760d1a762ce95f120a544970fcb32b476aacf584ef81779a29
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ccc(-c2cn[nH]c2)cc1
Br-[CH2;D2;+0:1]-[C:2]-[C:3]-[C:4](-[#8:5])=[O;D1;H0:6].[#7;a:7]1:[c:8]:[c:9]:[c:10]:[nH;D2;+0:11]:1>>[#8:5]-[C:4](=[O;D1;H0:6])-[C:3]-[C:2]-[CH2;D2;+0:1]-[n;H0;D3;+0:11]1:[#7;a:7]:[c:8]:[c:9]:[c:10]:1
52
[{"value": 52.0, "product": "C1(=CC=CC=C1)C=1C=NN(C1)CCCC(=O)OCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 13.8, "product": "C1(=CC=CC=C1)C=1C=NN(C1)CCCC(=O)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
The mixture of ethyl 4-bromobutyrate (0.400 g, 2.05 mmole), 4-phenyl-1H-pyrazole (0.296 g, 2.05 mmole) and K2CO3 (0.567 g, 4.10 mmole) in DMF (10 ml) was stirred at room temperature overnight. The reaction mixture was diluted with water (100 ml) and extracted with ethyl acetate (2×). The combined organic phases were wa...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1cn[nH]c1
c1cn[nH]c1
c1cn[nH]c1.c1ccccc1
HBr
O.CN(C)C=O
null
8
CCOC(=O)CCCBr.c1ccc(-c2cn[nH]c2)cc1>O.CN(C)C=O>CCOC(=O)CCCn1cc(-c2ccccc2)cn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-8caad14f2992442898e4732fb72846ce
CCOC(=O)CCCn1cc(-c2ccccc2)cn1>>O=C(O)CCCn1cc(-c2ccccc2)cn1
C1(=CC=CC=C1)C=1C=NN(C1)CCCC(=O)OCC.Cl>>C1(=CC=CC=C1)C=1C=NN(C1)CCCC(=O)O
CC[O:3][C:2](=[O:1])[CH2:4][CH2:5][CH2:6][n:7]1[cH:8][c:9](-[c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[cH:16][n:17]1>>[O:1]=[C:2]([OH:3])[CH2:4][CH2:5][CH2:6][n:7]1[cH:8][c:9](-[c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[cH:16][n:17]1
CCOC(=O)CCCn1cc(-c2ccccc2)cn1
O=C(O)CCCn1cc(-c2ccccc2)cn1
null
null
CO.[OH-].[Na+]
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(-c2cn[nH]c2)cc1
C-C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
78
[{"value": 78.0, "product": "C1(=CC=CC=C1)C=1C=NN(C1)CCCC(=O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 77.8, "product": "C1(=CC=CC=C1)C=1C=NN(C1)CCCC(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
A mixture of ethyl 4-(4-phenyl-1H-pyrazol-1-yl)butanoate (273 mg, 1.06 mmole) in methanol (5 ml) and 1N NaOH (5 mL) was stirred at room temperature for 2 hours. The reaction mixture was adjusted to be acidic (pH=3-4) with 6 N HCl with an ice bath and then extracted with EtOAc (3×). The combined organic phases were wash...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1cn[nH]c1.c1ccccc1
Other
CO.[OH-].[Na+]
null
2
CCOC(=O)CCCn1cc(-c2ccccc2)cn1>CO.[OH-].[Na+]>O=C(O)CCCn1cc(-c2ccccc2)cn1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9d67097666cd49fda27b3a9639fe655d
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=C(O)CCCn1cc(-c2ccccc2)cn1>>CCCCCn1/c(=N/NC(=O)CCCn2cc(-c3ccccc3)cn2)[nH]c(=O)c2[nH]cnc21
C1(=CC=CC=C1)C=1C=NN(C1)CCCC(=O)O.C(CCCC)N1/C(/NC(C=2NC=NC12)=O)=N/N.F[P-](F)(F)(F)(F)F.N1(N=NC2=C1C=CC=C2)O[P+](N(C)C)(N(C)C)N(C)C.C(C)N(CC)CC>>O=C1C=2NC=NC2N(\C(\N1)=N\NC(CCCN1N=CC(=C1)C1=CC=CC=C1)=O)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1/[c:7](=[N:8]/[NH2:9])[nH:26][c:27](=[O:28])[c:29]2[nH:30][cH:31][n:32][c:33]12.O[C:10](=[O:11])[CH2:12][CH2:13][CH2:14][n:15]1[cH:16][c:17](-[c:18]2[cH:19][cH:20][cH:21][cH:22][cH:23]2)[cH:24][n:25]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1/[c:7](=[N:8]/[NH:9][C:10](=[O:11])[...
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=C(O)CCCn1cc(-c2ccccc2)cn1
CCCCCn1/c(=N/NC(=O)CCCn2cc(-c3ccccc3)cn2)[nH]c(=O)c2[nH]cnc21
null
null
CN(C)C=O.CCOC(=O)C
Acylation
Carboxylic acid with primary amine to amide
e50d935ef072f0718d4e131af3df793f26e2f0a63884801973739584ab6e55ba
2740512737e2508c1c8d407d0ee271fd1e1c46ad16223e8e2fc1e12936af0dea
O=C(CCCn1cc(-c2ccccc2)cn1)N/N=c1\[nH]c(=O)c2[nH]cnc2[nH]1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4].[#7;a:5]/[c:6](=[#7:7]\[NH2;D1;+0:8]):[#7;a:9]>>[#7;a:5]/[c:6](=[#7:7]\[NH;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4]):[#7;a:9]
99.7
[{"value": 99.7, "product": "O=C1C=2NC=NC2N(\\C(\\N1)=N\\NC(CCCN1N=CC(=C1)C1=CC=CC=C1)=O)CCCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 99.7, "product": "O=C1C=2NC=NC2N(\\C(\\N1)=N\\NC(CCCN1N=CC(=C1)C1=CC=CC=C1)=O)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
A mixture of 4-(4-phenyl-1H-pyrazol-1-yl)butanoic acid (190 mg, 0.825 mmol), (2E)-3-pentyl-3,7-dihydro-1H-purine-2,6-dione 2-hydrazone (195.0 mg, 0.825 mmol), benzotriazol-1-yloxytris(dimethylamino)phosphonium hexafluorophosphate (401 mg, 0.908 mmol) and triethyl amine (0.23 ml, 1.65 mmol) in DMF (10 ml) was stirred at...
10.6084/m9.figshare.5104873.v1
null
Hydrazone.Carboxylic acid
Hydrazone amide
null
null
c1cn[nH]c1.c1ccccc1.c1ncc2[nH]cnc2n1
HO-
CN(C)C=O.CCOC(=O)C
null
8
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=C(O)CCCn1cc(-c2ccccc2)cn1>CN(C)C=O.CCOC(=O)C>CCCCCn1/c(=N/NC(=O)CCCn2cc(-c3ccccc3)cn2)[nH]c(=O)c2[nH]cnc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6add9091aa554342a6b67c226dcccd55
CCCCCn1/c(=N/NC(=O)CCCn2cc(-c3ccccc3)cn2)[nH]c(=O)c2[nH]cnc21>>CCCCCn1c2nc[nH]c2c(=O)n2c(CCCn3cc(-c4ccccc4)cn3)nnc12
O=C1C=2NC=NC2N(\C(\N1)=N\NC(CCCN1N=CC(=C1)C1=CC=CC=C1)=O)CCCCC>>C(CCCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)CCCN2N=CC(=C2)C2=CC=CC=C2
O=[C:15]([CH2:16][CH2:17][CH2:18][n:19]1[cH:20][c:21](-[c:22]2[cH:23][cH:24][cH:25][cH:26][cH:27]2)[cH:28][n:29]1)[NH:30]/[N:31]=[c:32]1/[n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[nH:14]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13...
CCCCCn1/c(=N/NC(=O)CCCn2cc(-c3ccccc3)cn2)[nH]c(=O)c2[nH]cnc21
CCCCCn1c2nc[nH]c2c(=O)n2c(CCCn3cc(-c4ccccc4)cn3)nnc12
null
null
C1(=CC=CC=C1)C
Aromatic Heterocycle Formation
OtherReaction
f919762557f16e8feb47c1fb62f203cd1ec4ed5f009cf276d2d0e0ec84ef6b80
78b0616e5760c6d4dadfc1fac5c58c0254d0dc7b1bf102fea4bc1349928b0776
O=c1c2[nH]cnc2[nH]c2nnc(CCCn3cc(-c4ccccc4)cn3)n12
O=[C;H0;D3;+0:1](-[C:2]-[C:3])-[NH;D2;+0:4]/[N;H0;D2;+0:5]=[c;H0;D3;+0:6]1\[nH;D2;+0:7]:[c:8](=[O;D1;H0:9]):[c:10]2:[#7;a:11]:[c:12]:[#7;a:13]:[c:14]:2:[#7;a:15]:1-[C:16]>>[C:3]-[C:2]-[c;H0;D3;+0:1]1:[n;H0;D2;+0:4]:[n;H0;D2;+0:5]:[c;H0;D3;+0:6]2:[#7;a:15](-[C:16]):[c:14]3:[#7;a:13]:[c:12]:[#7;a:11]:[c:10]:3:[c:8](=[O;D...
66
[{"value": 66.0, "product": "C(CCCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)CCCN2N=CC(=C2)C2=CC=CC=C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 66.0, "product": "C(CCCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)CCCN2N=CC(=C2)C2=CC=CC=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of N′-[(2E)-6-oxo-3-pentyl-1,3,6,7-tetrahydro-2H-purin-2-ylidene]-4-(4-phenyl-1H-pyrazol-1-yl)butanohydrazide (369 mg, 0.823 mmols) in toluene (20 ml) was refluxed for 2 hours. After cooling to room temperature, the solid formed was filtered, washed with EtOAc/Hexane (1:9) and dried to give the desired produc...
10.6084/m9.figshare.5104873.v1
null
Hydrazone amide
null
c1ncc2nc[nH]c2n1
c1nc2cn3cnnc3nc2[nH]1
c1cn[nH]c1.c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
HO-
C1(=CC=CC=C1)C
null
null
CCCCCn1/c(=N/NC(=O)CCCn2cc(-c3ccccc3)cn2)[nH]c(=O)c2[nH]cnc21>C1(=CC=CC=C1)C>CCCCCn1c2nc[nH]c2c(=O)n2c(CCCn3cc(-c4ccccc4)cn3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-eb3b578650aa424188ad18c782068849
CCCCCn1c2nc[nH]c2c(=O)n2c(CCCn3cc(-c4ccccc4)cn3)nnc12.O=C1CCC(=O)N1Br>>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCCn3cc(-c4ccccc4)cn3)nnc12
C(CCCC)N1C=2N(C(C=3NC=NC13)=O)C(=NN2)CCCN2N=CC(=C2)C2=CC=CC=C2.BrN1C(CCC1=O)=O>>BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CCCN3N=CC(=C3)C3=CC=CC=C3)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([CH2:17][CH2:18][CH2:19][n:20]3[cH:21][c:22](-[c:23]4[cH:24][cH:25][cH:26][cH:27][cH:28]4)[cH:29][n:30]3)[n:31][n:32][c:33]12.O=C1CCC(=O)N1[Br:10]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:1...
CCCCCn1c2nc[nH]c2c(=O)n2c(CCCn3cc(-c4ccccc4)cn3)nnc12.O=C1CCC(=O)N1Br
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCCn3cc(-c4ccccc4)cn3)nnc12
null
null
C1CCOC1
Functional Group Interconversion
Bromination
ec99ea20e93d70158a8c5b88a0324c2920957b29ee02a6abc4d48c347d7daa1b
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=c1c2[nH]cnc2[nH]c2nnc(CCCn3cc(-c4ccccc4)cn3)n12
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[cH;D2;+0:9]:[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]>>[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[c;H0;D3;+0:9](-[Br;H0;D1;+0:1]):[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]
38.3
[{"value": 38.0, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CCCN3N=CC(=C3)C3=CC=CC=C3)CCCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 38.3, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CCCN3N=CC(=C3)C3=CC=CC=C3)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
70
CELSIUS
1
HOUR
To a solution of 9-pentyl-3-[3-(4-phenyl-1H-pyrazol-1-yl)propyl]-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-5-one (234 mg, 0.543 mmol) in THF (45 ml) at room temperature was added N-bromosuccinimide (145 mg, 0.814 mmol). After stirring at 70° C. for 1 hour, the reaction mixture was concentrated and then purified by pre...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1nc2cn3cnnc3nc2[nH]1.C1CCNC1
c1nc2cn3cnnc3nc2[nH]1
c1cn[nH]c1.c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
HO-
C1CCOC1
70
1
CCCCCn1c2nc[nH]c2c(=O)n2c(CCCn3cc(-c4ccccc4)cn3)nnc12.O=C1CCC(=O)N1Br>C1CCOC1>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCCn3cc(-c4ccccc4)cn3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a302dec015f0498c9b6d3a146f377c91
CCOC(CCC#N)OCC.NO>>CCOC(CCC(=N)NO)OCC
C(C)OC(CCC#N)OCC.Cl.NO.C([O-])(O)=O.[Na+]>>C(C)OC(CCC(NO)=N)OCC
[CH3:1][CH2:2][O:3][CH:4]([CH2:5][CH2:6][C:7]#[N:8])[O:11][CH2:12][CH3:13].[NH2:9][OH:10]>>[CH3:1][CH2:2][O:3][CH:4]([CH2:5][CH2:6][C:7](=[NH:8])[NH:9][OH:10])[O:11][CH2:12][CH3:13]
CCOC(CCC#N)OCC.NO
CCOC(CCC(=N)NO)OCC
null
null
CO
Heteroatom Alkylation and Arylation
N-hydroxyimidamide from nitrile and hydroxylamine
08a01a2d1cd9346f7b3dddbfcbf8124b349e5763794287a4a1b9ee287b4d6aa7
38c3b778e04536ea6155ce05fc7c4746354a32b3703099defb07490833e3a961
null
[C:1]-[C:2]-[C;H0;D2;+0:3]#[N;H0;D1;+0:4].[NH2;D1;+0:5]-[O;D1;H1:6]>>[C:1]-[C:2]-[C;H0;D3;+0:3](=[NH;D1;+0:4])-[NH;D2;+0:5]-[O;D1;H1:6]
null
[]
null
null
null
null
A mixture of 4,4-diethoxybutanenitrile (5.0 g, 32 mmol), hydroxylamine hydrochloride (2.4 g, 35 mmol) and sodium bicarbonate (2.9 g, 35 mmol) in methanol (50 mL) was refluxed for 5 hours. After cooling to room temperature, the reaction mixture was concentrated and the residue was diluted with EtOAc and water. The water...
10.6084/m9.figshare.5104873.v1
null
Nitrile.Primary amine
Secondary amine
null
null
null
null
CO
null
null
CCOC(CCC#N)OCC.NO>CO>CCOC(CCC(=N)NO)OCC
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0ffafafad429422ba97c1c4487ecc9de
COc1ccc(-c2nc(CCC=O)no2)cc1.NN=C1N=C2N=CN=C2C(=O)N1>>CCCCCn1c2nc[nH]c2c(=O)n2c(CCc3noc(-c4ccc(OC)cc4)n3)nnc12
N1C(N=C2N=CN=C2C1=O)=NN.COC1=CC=C(C=C1)C1=NC(=NO1)CCC=O>>COC1=CC=C(C=C1)C1=NC(=NO1)CCC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O
O=[CH:15][CH2:16][CH2:17][c:18]1[n:19][o:20][c:21](-[c:22]2[cH:1][cH:24][c:25]([O:26][CH3:27])[cH:28][cH:29]2)[n:30]1.[N:6]1=[C:7]2[N:8]=[CH:9][N:10]=[C:11]2[C:12](=[O:13])[NH:14][C:33]1=[N:32][NH2:31]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[n:14]2[c:15]([CH2:16][CH2:17]...
COc1ccc(-c2nc(CCC=O)no2)cc1.NN=C1N=C2N=CN=C2C(=O)N1
CCCCCn1c2nc[nH]c2c(=O)n2c(CCc3noc(-c4ccc(OC)cc4)n3)nnc12
null
null
C(C)O
Aromatic Heterocycle Formation
OtherReaction
415438373b6c89916fe944451ebcf68817e04ded21a5bf5b90912a794744bab3
e6db118b5f632ca02d9e1ba56495e2a40001ccce13c863dabe2bbdda22b66d26
O=c1c2[nH]cnc2[nH]c2nnc(CCc3noc(-c4ccccc4)n3)n12
O=[CH;D2;+0:1]-[C:2]-[C:3]-[c:4]1:[#7;a:5]:[#8;a:6]:[c:7](-[c;H0;D3;+0:8]2:[c:9]:[c:10]:[c:11](-[#8:12]):[cH;D2;+0:13]:[cH;D2;+0:14]:2):[#7;a:15]:1.[NH2;D1;+0:16]-[N;H0;D2;+0:17]=[C;H0;D3;+0:18]1-[N;H0;D2;+0:19]=[C;H0;D3;+0:20]2-[N;H0;D2;+0:21]=[CH;D2;+0:22]-[N;H0;D2;+0:23]=[C;H0;D3;+0:24]-2-[C;H0;D3;+0:25](=[O;D1;H0:2...
95.4
[{"value": 64.0, "product": "COC1=CC=C(C=C1)C1=NC(=NO1)CCC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 95.4, "product": "COC1=CC=C(C=C1)C1=NC(=NO1)CCC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 1H-purine-2,6-dione 2-hydrazone (680 mg, 2.88 mmol) and 3-[5-(4-methoxyphenyl)-1,2,4-oxadiazol-3-yl]propanal (900 mg, 3.88 mmol) in ethanol (20 mL) was refluxed for 4 hours. The reaction mixture was concentrated and the residue was mixed with acetic acid (10 mL). The resulting mixture was refluxed for 3 ho...
10.6084/m9.figshare.5104873.v1
null
Hydrazone.Aldehyde.Substituted imine.Secondary amide
null
c1ccccc1.C1=NC2=NCNCC2=N1
c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
c1ncon1.c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
null
C(C)O
null
null
COc1ccc(-c2nc(CCC=O)no2)cc1.NN=C1N=C2N=CN=C2C(=O)N1>C(C)O>CCCCCn1c2nc[nH]c2c(=O)n2c(CCc3noc(-c4ccc(OC)cc4)n3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-6eb5ef580e5a4a8f893463dc31a9c088
CCCCCn1c2nc[nH]c2c(=O)n2c(CCc3noc(-c4ccc(OC)cc4)n3)nnc12.O=C1CCC(=O)N1Br>>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCc3noc(-c4ccc(OC)cc4)n3)nnc12
COC1=CC=C(C=C1)C1=NC(=NO1)CCC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O.BrN1C(CCC1=O)=O>>BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CCC3=NOC(=N3)C3=CC=C(C=C3)OC)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([CH2:17][CH2:18][c:19]3[n:20][o:21][c:22](-[c:23]4[cH:24][cH:25][c:26]([O:27][CH3:28])[cH:29][cH:30]4)[n:31]3)[n:32][n:33][c:34]12.O=C1CCC(=O)N1[Br:10]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])...
CCCCCn1c2nc[nH]c2c(=O)n2c(CCc3noc(-c4ccc(OC)cc4)n3)nnc12.O=C1CCC(=O)N1Br
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCc3noc(-c4ccc(OC)cc4)n3)nnc12
null
null
CN(C)C=O
Functional Group Interconversion
Bromination
ec99ea20e93d70158a8c5b88a0324c2920957b29ee02a6abc4d48c347d7daa1b
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=c1c2[nH]cnc2[nH]c2nnc(CCc3noc(-c4ccccc4)n3)n12
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[cH;D2;+0:9]:[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]>>[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[c;H0;D3;+0:9](-[Br;H0;D1;+0:1]):[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]
null
[]
70
CELSIUS
1
HOUR
To a solution of 3-2-[5-(4-methoxyphenyl)-1,2,4-oxadiazol-3-yl]ethyl-9-pentyl-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-5-one (160 mg, 0.36 mmol) in DMF (15 mL) at room temperature was added N-bromosuccinimide (110 mg, 0.61 mmol). After stirring at 70° C. for 1 hour, the reaction mixture was concentrated and purified ...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1nc2cn3cnnc3nc2[nH]1.C1CCNC1
c1nc2cn3cnnc3nc2[nH]1
c1ncon1.c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
HO-
CN(C)C=O
70
1
CCCCCn1c2nc[nH]c2c(=O)n2c(CCc3noc(-c4ccc(OC)cc4)n3)nnc12.O=C1CCC(=O)N1Br>CN(C)C=O>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCc3noc(-c4ccc(OC)cc4)n3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ee410f0fc6fe409099a58bd6e12bfbf4
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCc3noc(-c4ccc(OC)cc4)n3)nnc12>>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCc3noc(-c4ccc(O)cc4)n3)nnc12
BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CCC3=NOC(=N3)C3=CC=C(C=C3)OC)CCCCC.B(Br)(Br)Br>>BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CCC3=NOC(=N3)C3=CC=C(C=C3)O)CCCCC
C[O:27][c:26]1[cH:25][cH:24][c:23](-[c:22]2[o:21][n:20][c:19]([CH2:18][CH2:17][c:16]3[n:15]4[c:13](=[O:14])[c:12]5[c:7]([n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:33]4[n:32][n:31]3)[n:8][c:9]([Br:10])[nH:11]5)[n:30]2)[cH:29][cH:28]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:11][c:12]2[c:1...
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCc3noc(-c4ccc(OC)cc4)n3)nnc12
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCc3noc(-c4ccc(O)cc4)n3)nnc12
null
null
C(Cl)Cl
Deprotection
Cleavage of methoxy ethers to alcohols
c5320c7dfa4f544d4900efcae9b3262bf0d5286bcf39c86109232351f35b23d5
26a36596df80ec137b0e8087297418351c93c32819177f680675220622f215d4
O=c1c2[nH]cnc2[nH]c2nnc(CCc3noc(-c4ccccc4)n3)n12
C-[O;H0;D2;+0:1]-[c:2](:[c:3]):[c:4]>>[OH;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
8
HOUR
To a solution of 7-bromo-3-2-[5-(4-methoxyphenyl)-1,2,4-oxadiazol-3-yl]ethyl-9-pentyl-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-5-one (190 mg, 0.36 mmol) in CH2Cl2 (12 mL) was added a solution of BBr3 in CH2Cl2 (1 M, 7.0 ml, 7.0 mmol) at room temperature. After stirring at room temperature overnight, the reaction mixt...
10.6084/m9.figshare.5104873.v1
null
Ether
Aromatic alcohol
null
null
c1ncon1.c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
Other
C(Cl)Cl
null
8
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCc3noc(-c4ccc(OC)cc4)n3)nnc12>C(Cl)Cl>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCc3noc(-c4ccc(O)cc4)n3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-ea40a2eea40b4c0abae5aec9b060ced3
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=CCCNC(=O)OCc1ccccc1>>CCCCCn1/c(=N/N=C\CCNC(=O)OCc2ccccc2)[nH]c(=O)c2[nH]cnc21
C(CCCC)N1/C(/NC(C=2NC=NC12)=O)=N/N.O=CCCNC(OCC1=CC=CC=C1)=O>>O=C1C=2NC=NC2N(\C(\N1)=N\N=C/CCNC(OCC1=CC=CC=C1)=O)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1/[c:7](=[N:8]/[NH2:9])[nH:24][c:25](=[O:26])[c:27]2[nH:28][cH:29][n:30][c:31]12.O=[CH:10][CH2:11][CH2:12][NH:13][C:14](=[O:15])[O:16][CH2:17][c:18]1[cH:19][cH:20][cH:21][cH:22][cH:23]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1/[c:7](=[N:8]/[N:9]=[CH:10]\[CH2:11][CH2:12][NH:13][...
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=CCCNC(=O)OCc1ccccc1
CCCCCn1/c(=N/N=C\CCNC(=O)OCc2ccccc2)[nH]c(=O)c2[nH]cnc21
null
null
C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
369b3f62a39edf615315b2761263eb1b649612c7b3caef083e9b41e01b478de5
a492f13607987389cdd7ab2f9f1199c71d7d1e56ec2df1828d06f8b8bbe23769
O=C(NCC/C=N\N=c1/[nH]c(=O)c2[nH]cnc2[nH]1)OCc1ccccc1
O=[CH;D2;+0:1]-[C:2]-[C:3].[#7;a:4]/[c:5](=[#7:6]\[NH2;D1;+0:7]):[#7;a:8]>>[#7;a:4]/[c:5](=[#7:6]\[N;H0;D2;+0:7]=[CH;D2;+0:1]/[C:2]-[C:3]):[#7;a:8]
97.9
[{"value": 58.0, "product": "O=C1C=2NC=NC2N(\\C(\\N1)=N\\N=C/CCNC(OCC1=CC=CC=C1)=O)CCCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 97.9, "product": "O=C1C=2NC=NC2N(\\C(\\N1)=N\\N=C/CCNC(OCC1=CC=CC=C1)=O)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of (2E)-3-pentyl-3,7-dihydro-1H-purine-2,6-dione 2-hydrazone (2.3 g, 9.6 mmol) and benzyl (3-oxopropyl)carbamate (2.0 g, 9.6 mmol) in ethanol (30 mL) was refluxed overnight. The reaction mixture was concentrated to give the product (4.0 g, 58% yield), which was used for next step without further purification....
10.6084/m9.figshare.5104873.v1
null
Hydrazone.Aldehyde
null
null
null
c1ccccc1.c1ncc2[nH]cnc2n1
HO-
C(C)O
null
null
CCCCCn1/c(=N/N)[nH]c(=O)c2[nH]cnc21.O=CCCNC(=O)OCc1ccccc1>C(C)O>CCCCCn1/c(=N/N=C\CCNC(=O)OCc2ccccc2)[nH]c(=O)c2[nH]cnc21
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-1d540088b85c478584e758869c1dcc48
CCCCCn1/c(=N/N=C\CCNC(=O)OCc2ccccc2)[nH]c(=O)c2[nH]cnc21>>CCCCCn1c2nc[nH]c2c(=O)n2c(CCNC(=O)OCc3ccccc3)nnc12
O=C1C=2NC=NC2N(\C(\N1)=N\N=C/CCNC(OCC1=CC=CC=C1)=O)CCCCC>>O=C1C=2NC=NC2N(C=2N1C(=NN2)CCNC(OCC2=CC=CC=C2)=O)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[nH:14]/[c:31]1=[N:30]\[N:29]=[CH:15]/[CH2:16][CH2:17][NH:18][C:19](=[O:20])[O:21][CH2:22][c:23]1[cH:24][cH:25][cH:26][cH:27][cH:28]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[n:14]2[c:1...
CCCCCn1/c(=N/N=C\CCNC(=O)OCc2ccccc2)[nH]c(=O)c2[nH]cnc21
CCCCCn1c2nc[nH]c2c(=O)n2c(CCNC(=O)OCc3ccccc3)nnc12
null
null
C(C)(=O)O
Aromatic Heterocycle Formation
OtherReaction
066077903128dcf5e3d8c17f71c894783195993eb8e78fea83753934f8800b97
42048ba06e684767e79a864f38d2ee087b4547e971032cda3c892dd210eef093
O=C(NCCc1nnc2[nH]c3nc[nH]c3c(=O)n12)OCc1ccccc1
[C:1]-[C:2]/[CH;D2;+0:3]=[N;H0;D2;+0:4]\[N;H0;D2;+0:5]=[c;H0;D3;+0:6]1/[nH;D2;+0:7]:[c:8](=[O;D1;H0:9]):[c:10]2:[#7;a:11]:[c:12]:[#7;a:13]:[c:14]:2:[#7;a:15]:1-[C:16]>>[C:1]-[C:2]-[c;H0;D3;+0:3]1:[n;H0;D2;+0:4]:[n;H0;D2;+0:5]:[c;H0;D3;+0:6]2:[#7;a:15](-[C:16]):[c:14]3:[#7;a:13]:[c:12]:[#7;a:11]:[c:10]:3:[c:8](=[O;D1;H0...
54.8
[{"value": 54.0, "product": "O=C1C=2NC=NC2N(C=2N1C(=NN2)CCNC(OCC2=CC=CC=C2)=O)CCCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 54.8, "product": "O=C1C=2NC=NC2N(C=2N1C(=NN2)CCNC(OCC2=CC=CC=C2)=O)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of benzyl (3Z)-3-[(2E)-(6-oxo-3-pentyl-1,3,6,7-tetrahydro-2H-purin-2-ylidene)hydrazono]propylcarbamate (4.0 g, 5.6 mmol) in acetic acid (50 mL) was refluxed in the air overnight. The mixture was concentrated and purified by preparative LCMS to give the desired product (1.3 g, 54% yield) as a white solid. LCMS...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ncc2nc[nH]c2n1
c1nc2cn3cnnc3nc2[nH]1
c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
null
C(C)(=O)O
null
null
CCCCCn1/c(=N/N=C\CCNC(=O)OCc2ccccc2)[nH]c(=O)c2[nH]cnc21>C(C)(=O)O>CCCCCn1c2nc[nH]c2c(=O)n2c(CCNC(=O)OCc3ccccc3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-fa626a7c0a53495abf1710c96a707653
CCCCCn1c2nc[nH]c2c(=O)n2c(CCNC(=O)OCc3ccccc3)nnc12>>CCCCCn1c2nc[nH]c2c(=O)n2c(CCN)nnc12
O=C1C=2NC=NC2N(C=2N1C(=NN2)CCNC(OCC2=CC=CC=C2)=O)CCCCC>>NCCC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O
O=C(OCc1ccccc1)[NH:18][CH2:17][CH2:16][c:15]1[n:14]2[c:12](=[O:13])[c:11]3[c:7]([n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:21]2[n:20][n:19]1)[n:8][cH:9][nH:10]3>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:10][c:11]2[c:12](=[O:13])[n:14]2[c:15]([CH2:16][CH2:17][NH2:18])[n:19][n:20][c:21]12
CCCCCn1c2nc[nH]c2c(=O)n2c(CCNC(=O)OCc3ccccc3)nnc12
CCCCCn1c2nc[nH]c2c(=O)n2c(CCN)nnc12
null
[Pd]
CO
Reduction
Hydrogenolysis of amides/imides/carbamates
087b6600ba91d3df931fe6979f2445c192cbfd59e04fd2d8a10f7c7573ac669f
4e549866ec1acadec4c84aaf8495992a28ec78d8ea5ef1b9f44dd843b0dcb7d4
O=c1c2[nH]cnc2[nH]c2nncn12
O=C(-O-C-c1:c:c:c:c:c:1)-[NH;D2;+0:1]-[C:2]-[C:3]>>[C:3]-[C:2]-[NH2;D1;+0:1]
92.2
[{"value": 90.0, "product": "NCCC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 92.2, "product": "NCCC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of benzyl [2-(5-oxo-9-pentyl-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-3-yl)ethyl]carbamate (0.52 g, 1.2 mmol) in methanol (50 mL) was added 10% Pd/C (100 mg). The reaction mixture was shaken in a hydrogenation reactor under 50 Psi H2 for 3 hours. The reaction mixture was filtered through a pad of celite...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether
Primary amine
c1ccccc1
null
c1nc2cn3cnnc3nc2[nH]1
HO-
[Pd].CO
null
null
CCCCCn1c2nc[nH]c2c(=O)n2c(CCNC(=O)OCc3ccccc3)nnc12>[Pd].CO>CCCCCn1c2nc[nH]c2c(=O)n2c(CCN)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-30bcb777201b43de839009bee00a8066
CCCCCn1c2nc[nH]c2c(=O)n2c(CCN)nnc12.O=C1CCC(=O)N1Br>>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCN)nnc12
NCCC1=NN=C2N1C(C=1NC=NC1N2CCCCC)=O.BrN1C(CCC1=O)=O>>NCCC1=NN=C2N1C(C=1NC(=NC1N2CCCCC)Br)=O
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][cH:9][nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([CH2:17][CH2:18][NH2:19])[n:20][n:21][c:22]12.O=C1CCC(=O)N1[Br:10]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([CH2:17][CH2:18][NH2:19])[n:20][n:21][c:22...
CCCCCn1c2nc[nH]c2c(=O)n2c(CCN)nnc12.O=C1CCC(=O)N1Br
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCN)nnc12
null
null
C1CCOC1
Functional Group Interconversion
Bromination
ec99ea20e93d70158a8c5b88a0324c2920957b29ee02a6abc4d48c347d7daa1b
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=c1c2[nH]cnc2[nH]c2nncn12
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[cH;D2;+0:9]:[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]>>[#7;a:2]:[#7;a:3]:[c:4]1:[#7;a:5]:[c:6]:[c:7]2:[#7;a:8]:[c;H0;D3;+0:9](-[Br;H0;D1;+0:1]):[#7;a:10]:[c:11]:2:[#7;a:12]:1-[C:13]
76
[{"value": 76.0, "product": "NCCC1=NN=C2N1C(C=1NC(=NC1N2CCCCC)Br)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 74.1, "product": "NCCC1=NN=C2N1C(C=1NC(=NC1N2CCCCC)Br)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
70
CELSIUS
1
HOUR
To a mixture of 3-(2-aminoethyl)-9-pentyl-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-5-one (310 mg, 1.1 mmol) in THF (50 mL), was added N-Bromosuccinimide (0.29 g, 1.6 mmol). The mixture was stirred at 70° C. for 1 hour. The reaction mixture was concentrated. The solid was filtered and washed with EtOAc to yield the de...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1nc2cn3cnnc3nc2[nH]1.C1CCNC1
c1nc2cn3cnnc3nc2[nH]1
c1nc2cn3cnnc3nc2[nH]1
HO-
C1CCOC1
70
1
CCCCCn1c2nc[nH]c2c(=O)n2c(CCN)nnc12.O=C1CCC(=O)N1Br>C1CCOC1>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCN)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-fc36eedd2d934f338ea7fb8ac31ec2ef
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCN)nnc12.COc1ccc(C(=O)O)cc1>>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCNC(=O)c3ccc(OC)cc3)nnc12
NCCC1=NN=C2N1C(C=1NC(=NC1N2CCCCC)Br)=O.COC1=CC=C(C(=O)O)C=C1.F[P-](F)(F)(F)(F)F.N1(N=NC2=C1C=CC=C2)O[P+](N(C)C)(N(C)C)N(C)C.C(C)N(CC)CC>>BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CCNC(C3=CC=C(C=C3)OC)=O)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([CH2:17][CH2:18][NH2:19])[n:30][n:31][c:32]12.O[C:20](=[O:21])[c:22]1[cH:23][cH:24][c:25]([O:26][CH3:27])[cH:28][cH:29]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:11][c:12]2[c:13](=[...
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCN)nnc12.COc1ccc(C(=O)O)cc1
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCNC(=O)c3ccc(OC)cc3)nnc12
null
null
O.C(C)#N.CN(C)C=O
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(NCCc1nnc2[nH]c3nc[nH]c3c(=O)n12)c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C:6]-[C:7]-[NH2;D1;+0:8]>>[C:6]-[C:7]-[NH;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
73
[{"value": 73.0, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CCNC(C3=CC=C(C=C3)OC)=O)CCCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 69.7, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CCNC(C3=CC=C(C=C3)OC)=O)CCCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
A mixture of 3-(2-aminoethyl)-7-bromo-9-pentyl-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-5-one (70 mg, 0.20 mmol), 4-methoxybenzoic acid (32 mg, 0.21 mmol), benzotriazol-1-yloxytris(dimethylamino)phosphonium hexafluorophosphate (92 mg, 0.21 mmol), and triethylamine (0.053 mL, 0.38 mmol) in DMF (5 mL) was stirred at ro...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
HO-
O.C(C)#N.CN(C)C=O
null
8
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCN)nnc12.COc1ccc(C(=O)O)cc1>O.C(C)#N.CN(C)C=O>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCNC(=O)c3ccc(OC)cc3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-18d292e8812a4a5cbb73d639cd1ee844
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCN)nnc12.O=C=Nc1ccccc1>>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCNC(=O)Nc3ccccc3)nnc12
NCCC1=NN=C2N1C(C=1NC(=NC1N2CCCCC)Br)=O.C1(=CC=CC=C1)N=C=O>>BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CCNC(=O)NC3=CC=CC=C3)CCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:11][c:12]2[c:13](=[O:14])[n:15]2[c:16]([CH2:17][CH2:18][NH2:19])[n:29][n:30][c:31]12.[C:20](=[O:21])=[N:22][c:23]1[cH:24][cH:25][cH:26][cH:27][cH:28]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:11][c:12]2[c:13](=[O:14])[n:...
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCN)nnc12.O=C=Nc1ccccc1
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCNC(=O)Nc3ccccc3)nnc12
null
null
O.C(C)#N.CN(C)C=O
Acylation
Urea synthesis via isocyanate and primary amine
d39cd7dc52a79bb265ff8ef61ef7bf9dc7f7b5fb0150fcb4881bdfb18ab9c380
a5dc801930c765d2a435a0a2973e50163c305ba8e7641d6adbcc1550b7b96de7
O=C(NCCc1nnc2[nH]c3nc[nH]c3c(=O)n12)Nc1ccccc1
[C:1]-[C:2]-[NH2;D1;+0:3].[O;D1;H0:4]=[C;H0;D2;+0:5]=[N;H0;D2;+0:6]-[c:7](:[c:8]):[c:9]>>[C:1]-[C:2]-[NH;D2;+0:3]-[C;H0;D3;+0:5](=[O;D1;H0:4])-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]
80
[{"value": 80.0, "product": "BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CCNC(=O)NC3=CC=CC=C3)CCCCC", "details": "PERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
A mixture of 3-(2-aminoethyl)-7-bromo-9-pentyl-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-5-one (62 mg, 0.17 mmol) and phenyl isocyanate (0.018 mL, 0.16 mmol) in DMF (5 mL) was stirred at room temperature overnight. The reaction mixture was diluted with water and acetonitrile and then purified by preparative LCMS to gi...
10.6084/m9.figshare.5104873.v1
null
Isocyanate.Primary amine
Urea
null
null
c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
null
O.C(C)#N.CN(C)C=O
null
8
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCN)nnc12.O=C=Nc1ccccc1>O.C(C)#N.CN(C)C=O>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCNC(=O)Nc3ccccc3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-f77f09454d8640f9bf014e4ad2eb415f
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCNC(=O)c3ccc(OC)cc3)nnc12>>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCNC(=O)c3ccc(O)cc3)nnc12
BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CCNC(C3=CC=C(C=C3)OC)=O)CCCCC.B(Br)(Br)Br>>BrC1=NC=2N(C=3N(C(C2N1)=O)C(=NN3)CCNC(C3=CC=C(C=C3)O)=O)CCCCC
C[O:26][c:25]1[cH:24][cH:23][c:22]([C:20]([NH:19][CH2:18][CH2:17][c:16]2[n:15]3[c:13](=[O:14])[c:12]4[c:7]([n:6]([CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])[c:31]3[n:30][n:29]2)[n:8][c:9]([Br:10])[nH:11]4)=[O:21])[cH:28][cH:27]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][n:6]1[c:7]2[n:8][c:9]([Br:10])[nH:11][c:12]2[c:13](=[O:14])[n...
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCNC(=O)c3ccc(OC)cc3)nnc12
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCNC(=O)c3ccc(O)cc3)nnc12
null
null
C(Cl)Cl
Deprotection
Cleavage of methoxy ethers to alcohols
c5320c7dfa4f544d4900efcae9b3262bf0d5286bcf39c86109232351f35b23d5
26a36596df80ec137b0e8087297418351c93c32819177f680675220622f215d4
O=C(NCCc1nnc2[nH]c3nc[nH]c3c(=O)n12)c1ccccc1
C-[O;H0;D2;+0:1]-[c:2](:[c:3]):[c:4]>>[OH;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
8
HOUR
To a solution of N-[2-(7-bromo-5-oxo-9-pentyl-6,9-dihydro-5H-[1,2,4]triazolo[4,3-a]purin-3-yl)ethyl]-4-methoxybenzamide (63.0 mg, 0.125 mmol) in CH2Cl2 (5 mL) at 0° C. was added a solution of Boron tribromide in CH2Cl2 (1.0 M, 1.3 mL, 1.3 mmol). The mixture was stirred at room temperature overnight. The reaction mixtur...
10.6084/m9.figshare.5104873.v1
null
Ether
Aromatic alcohol
null
null
c1ccccc1.c1nc2cn3cnnc3nc2[nH]1
Other
C(Cl)Cl
null
8
CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCNC(=O)c3ccc(OC)cc3)nnc12>C(Cl)Cl>CCCCCn1c2nc(Br)[nH]c2c(=O)n2c(CCNC(=O)c3ccc(O)cc3)nnc12
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-4ab0fe31746f4de89f022f8d6cc85a9d
CC(C)(N)CCn1cnnc1.CCOC(O)C(=O)c1ccc(OCc2ccccc2)c(C(=O)OC)c1>>COC(=O)c1cc(C(=O)C=NC(C)(C)CCn2cnnc2)ccc1OCc1ccccc1
C(C1=CC=CC=C1)OC1=C(C(=O)OC)C=C(C=C1)C(C(O)OCC)=O.CC(CCN1C=NN=C1)(C)N>>C(C1=CC=CC=C1)OC1=C(C(=O)OC)C=C(C=C1)C(C=NC(CCN1C=NN=C1)(C)C)=O
[NH2:11][C:12]([CH3:13])([CH3:14])[CH2:15][CH2:16][n:17]1[cH:18][n:19][n:20][cH:21]1.CCO[CH:10](O)[C:8]([c:7]1[cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[c:24]([O:25][CH2:26][c:27]2[cH:28][cH:29][cH:30][cH:31][cH:32]2)[cH:23][cH:22]1)=[O:9]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([C:8](=[O:9])[CH:10]=[N:11][C:12]([CH3:1...
CC(C)(N)CCn1cnnc1.CCOC(O)C(=O)c1ccc(OCc2ccccc2)c(C(=O)OC)c1
COC(=O)c1cc(C(=O)C=NC(C)(C)CCn2cnnc2)ccc1OCc1ccccc1
null
null
C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
9f630e6c2b6d7517a3fa7357236cf4ddfd17dba1b594cd96ae8996ff5f3995d6
62cc0e6b65becc601a2e48497b9a7abf308c36c68e35364f9fb60106ecf6b8b5
O=C(C=NCCCn1cnnc1)c1ccc(OCc2ccccc2)cc1
C-C-O-[CH;D3;+0:1](-O)-[C:2](=[O;D1;H0:3])-[c:4].[C:5]-[C:6](-[C;D1;H3:7])(-[C;D1;H3:8])-[NH2;D1;+0:9]>>[C:5]-[C:6](-[C;D1;H3:7])(-[C;D1;H3:8])-[N;H0;D2;+0:9]=[CH;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]
null
[]
null
null
null
null
16 g of methyl 2-benzyloxy-5-(2-ethoxy-2-hydroxy-acetyl)-benzoate and 6 g of 1,1-dimethyl-3-[1,2,4]triazol-4-yl-propylamine are heated to 70° C. for one hour in 100 mL ethanol. Then half the solvent is distilled off and the mixture remaining is cooled. The product that crystallises out is suction filtered and washed wi...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ether.Secondary alcohol.Primary amine
Ketone.Substituted imine
null
null
c1ccccc1.c1nnc[nH]1.c1ccccc1
HO-
C(C)O
null
null
CC(C)(N)CCn1cnnc1.CCOC(O)C(=O)c1ccc(OCc2ccccc2)c(C(=O)OC)c1>C(C)O>COC(=O)c1cc(C(=O)C=NC(C)(C)CCn2cnnc2)ccc1OCc1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-25c24f0e1d404431b21b22ec9c290112
COC(=O)c1cc(C(=O)CNC(C)(C)CCn2cnnc2)ccc1OCc1ccccc1>>CC(C)(CCn1cnnc1)NCC(O)c1ccc(OCc2ccccc2)c(CO)c1
CC(=O)C.[Cl-].[Ca+2].[Cl-].C(C1=CC=CC=C1)OC1=C(C(=O)OC)C=C(C=C1)C(CNC(CCN1C=NN=C1)(C)C)=O.[BH4-].[Na+]>>C(C1=CC=CC=C1)OC1=C(C=C(C=C1)C(CNC(CCN1C=NN=C1)(C)C)O)CO
CO[C:28]([c:27]1[c:18]([O:19][CH2:20][c:21]2[cH:22][cH:23][cH:24][cH:25][cH:26]2)[cH:17][cH:16][c:15]([C:13]([CH2:12][NH:11][C:2]([CH3:1])([CH3:3])[CH2:4][CH2:5][n:6]2[cH:7][n:8][n:9][cH:10]2)=[O:14])[cH:30]1)=[O:29]>>[CH3:1][C:2]([CH3:3])([CH2:4][CH2:5][n:6]1[cH:7][n:8][n:9][cH:10]1)[NH:11][CH2:12][CH:13]([OH:14])[c:1...
COC(=O)c1cc(C(=O)CNC(C)(C)CCn2cnnc2)ccc1OCc1ccccc1
CC(C)(CCn1cnnc1)NCC(O)c1ccc(OCc2ccccc2)c(CO)c1
null
null
O1CCCC1.C(C)(=O)O.C(C)O
Reduction
OtherReaction
67089bd4b5ba61d4201285032d065b7dbb074f27b1058a42daae9f0677a26309
fb0acaa903b6e5b1d95989a91fad01e909b2ecc65b96c636622bf14cc20a64c2
c1ccc(COc2ccc(CCNCCCn3cnnc3)cc2)cc1
C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3](:[c:4]):[c:5]:[c:6](-[C;H0;D3;+0:7](=[O;H0;D1;+0:8])-[C:9]-[#7:10]):[c:11]>>[#7:10]-[C:9]-[CH;D3;+0:7](-[OH;D1;+0:8])-[c:6](:[c:11]):[c:5]:[c:3](-[CH2;D2;+0:1]-[OH;D1;+0:2]):[c:4]
null
[]
5
CELSIUS
8
HOUR
5 g of calcium chloride are dissolved in 50 mL ethanol. Then 10 g of methyl 2-benzyloxy-5-[2-(1,1-dimethyl-3-[1,2,4]triazol-4-yl-propylamino)-acetyl]-benzoate in 100 mL tetrahydrofuran are added and the mixture is cooled to 5° C. It is combined batchwise with 3.5 g of sodium borohydride and stirred overnight while heat...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ester
Primary alcohol.Secondary alcohol
null
null
c1nnc[nH]1.c1ccccc1.c1ccccc1
Other
O1CCCC1.C(C)(=O)O.C(C)O
5
8
COC(=O)c1cc(C(=O)CNC(C)(C)CCn2cnnc2)ccc1OCc1ccccc1>O1CCCC1.C(C)(=O)O.C(C)O>CC(C)(CCn1cnnc1)NCC(O)c1ccc(OCc2ccccc2)c(CO)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-a6850de313434d4bbf3726e7f136eee8
CC(=O)OC(CNC(C)(C)CCn1cnnc1)c1ccc(OCc2ccccc2)c(CO)c1>>CC(C)(CCn1cnnc1)NCC(O)c1ccc(O)c(CO)c1
C(C)(=O)OC(CNC(CCN1C=NN=C1)(C)C)C1=CC(=C(C=C1)OCC1=CC=CC=C1)CO.[H][H]>>CC(CCN1C=NN=C1)(C)NCC(O)C1=CC(=C(C=C1)O)CO
CC(=O)[O:14][CH:13]([CH2:12][NH:11][C:2]([CH3:1])([CH3:3])[CH2:4][CH2:5][n:6]1[cH:7][n:8][n:9][cH:10]1)[c:15]1[cH:16][cH:17][c:18]([O:19]Cc2ccccc2)[c:20]([CH2:21][OH:22])[cH:23]1>>[CH3:1][C:2]([CH3:3])([CH2:4][CH2:5][n:6]1[cH:7][n:8][n:9][cH:10]1)[NH:11][CH2:12][CH:13]([OH:14])[c:15]1[cH:16][cH:17][c:18]([OH:19])[c:20]...
CC(=O)OC(CNC(C)(C)CCn1cnnc1)c1ccc(OCc2ccccc2)c(CO)c1
CC(C)(CCn1cnnc1)NCC(O)c1ccc(O)c(CO)c1
null
[Pd]
CO
Reduction
OtherReaction
5191c2a4aa54a541316ab8da2c23088325133ca5b0a78ef65048e93be8ca25c3
34ee45d408c5a96781b888def3a5f72b571220140037e25fd3d3fe11cbb09ec2
c1ccc(CCNCCCn2cnnc2)cc1
C-C(=O)-[O;H0;D2;+0:1]-[C:2](-[C:3])-[c:4].[c:5]:[c:6](-[O;H0;D2;+0:7]-C-c1:c:c:c:c:c:1):[c:8]>>[C:3]-[C:2](-[OH;D1;+0:1])-[c:4].[OH;D1;+0:7]-[c:6](:[c:5]):[c:8]
null
[]
null
null
null
null
5 g of 1-(4-benzyloxy-3-hydroxymethyl-phenyl)-2-(1,1-dimethyl-3-[1,2,4]triazol-4-yl-propylamino)-ethanol acetate are hydrogenated with 0.5 g of palladium on charcoal (5%) in 100 mL methanol. After the theoretically calculated amount of hydrogen has been taken up the catalyst is filtered off and the filtrate is evaporat...
10.6084/m9.figshare.5104873.v1
null
Ester.Ether
Secondary alcohol.Aromatic alcohol
c1ccccc1
null
c1nnc[nH]1.c1ccccc1
HO-
[Pd].CO
null
null
CC(=O)OC(CNC(C)(C)CCn1cnnc1)c1ccc(OCc2ccccc2)c(CO)c1>[Pd].CO>CC(C)(CCn1cnnc1)NCC(O)c1ccc(O)c(CO)c1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-9f34e6e3d751450c9ab46d4ded2de53c
CCOC(O)C(=O)c1ccc(OCc2ccccc2)c(C(=O)OC)c1.COc1ccc(-c2nc(C)n(CCC(C)(C)N)n2)cc1>>COC(=O)c1cc(C(O)CNC(C)(C)CCn2nc(-c3ccc(OC)cc3)nc2C)ccc1OCc1ccccc1
CC(=O)C.C(C1=CC=CC=C1)OC1=C(C(=O)OC)C=C(C=C1)C(C(O)OCC)=O.COC1=CC=C(C=C1)C1=NN(C(=N1)C)CCC(C)(C)N.[BH4-].[Na+]>>C(C1=CC=CC=C1)OC1=C(C(=O)OC)C=C(C=C1)C(CNC(CCN1N=C(N=C1C)C1=CC=C(C=C1)OC)(C)C)O
CCO[CH:10](O)[C:8]([c:7]1[cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[c:33]([O:34][CH2:35][c:36]2[cH:37][cH:38][cH:39][cH:40][cH:41]2)[cH:32][cH:31]1)=[O:9].[NH2:11][C:12]([CH3:13])([CH3:14])[CH2:15][CH2:16][n:17]1[n:18][c:19](-[c:20]2[cH:21][cH:22][c:23]([O:24][CH3:25])[cH:26][cH:27]2)[n:28][c:29]1[CH3:30]>>[CH3:1][O:2][C:3...
CCOC(O)C(=O)c1ccc(OCc2ccccc2)c(C(=O)OC)c1.COc1ccc(-c2nc(C)n(CCC(C)(C)N)n2)cc1
COC(=O)c1cc(C(O)CNC(C)(C)CCn2nc(-c3ccc(OC)cc3)nc2C)ccc1OCc1ccccc1
null
null
C(C)(=O)O.C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
1fdebd18d8e186352a5054d1639a246066c291a759c2941bdb27defc05ab0b96
270f718637e505454980bf4a24a04f3a3a166f4d4160855797b4e1923ac25b66
c1ccc(COc2ccc(CCNCCCn3cnc(-c4ccccc4)n3)cc2)cc1
C-C-O-[CH;D3;+0:1](-O)-[C;H0;D3;+0:2](=[O;H0;D1;+0:3])-[c:4](:[c:5]):[c:6].[C:7]-[C:8](-[C;D1;H3:9])(-[C;D1;H3:10])-[NH2;D1;+0:11]>>[C:7]-[C:8](-[C;D1;H3:9])(-[C;D1;H3:10])-[NH;D2;+0:11]-[CH2;D2;+0:1]-[CH;D3;+0:2](-[OH;D1;+0:3])-[c:4](:[c:5]):[c:6]
null
[]
10
CELSIUS
3
HOUR
8.5 g of methyl 2-benzyloxy-5-(2-ethoxy-2-hydroxy-acetyl)-benzoate and 4.9 g of 3-[3-(4-methoxy-phenyl)-5-methyl-[1,2,4]triazol-1-yl]-1,1-dimethyl-propylamine in 100 mL ethanol are stirred for three hours at 60° C., cooled to 10° C., combined batchwise with 0.8 g of sodium borohydride and stirred for a further three ho...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ether.Secondary alcohol.Primary amine
Secondary alcohol.Secondary amine
null
null
c1ccccc1.c1nc[nH]n1.c1ccccc1.c1ccccc1
HO-
C(C)(=O)O.C(C)O
10
3
CCOC(O)C(=O)c1ccc(OCc2ccccc2)c(C(=O)OC)c1.COc1ccc(-c2nc(C)n(CCC(C)(C)N)n2)cc1>C(C)(=O)O.C(C)O>COC(=O)c1cc(C(O)CNC(C)(C)CCn2nc(-c3ccc(OC)cc3)nc2C)ccc1OCc1ccccc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-d146b460d3904465aaaa50ff037c40c0
COc1ccc(-c2nc(C)n(CCC(C)(C)NCC(O)c3ccc(OCc4ccccc4)c(CO)c3)n2)cc1>>COc1ccc(-c2nc(C)n(CCC(C)(C)NCC(O)c3ccc(O)c(CO)c3)n2)cc1
C(C1=CC=CC=C1)OC1=C(C=C(C=C1)C(CNC(CCN1N=C(N=C1C)C1=CC=C(C=C1)OC)(C)C)O)CO>>OC(CNC(CCN1N=C(N=C1C)C1=CC=C(C=C1)OC)(C)C)C1=CC(=C(C=C1)O)CO
c1ccc(C[O:25][c:24]2[cH:23][cH:22][c:21]([CH:19]([CH2:18][NH:17][C:14]([CH2:13][CH2:12][n:11]3[c:9]([CH3:10])[n:8][c:7](-[c:6]4[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:32][cH:31]4)[n:30]3)([CH3:15])[CH3:16])[OH:20])[cH:29][c:26]2[CH2:27][OH:28])cc1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[n:8][c:9]([CH3:10])[n:11]([CH2:1...
COc1ccc(-c2nc(C)n(CCC(C)(C)NCC(O)c3ccc(OCc4ccccc4)c(CO)c3)n2)cc1
COc1ccc(-c2nc(C)n(CCC(C)(C)NCC(O)c3ccc(O)c(CO)c3)n2)cc1
null
[Pd]
CO
Deprotection
Hydroxyl benzyl deprotection
36869d1fe85185a14d9eb30bf05178c600a9b6eca277ffaf3803578c30e0bf5d
26a36596df80ec137b0e8087297418351c93c32819177f680675220622f215d4
c1ccc(CCNCCCn2cnc(-c3ccccc3)n2)cc1
[c:1]:[c:2](-[O;H0;D2;+0:3]-C-c1:c:c:c:c:c:1):[c:4]>>[OH;D1;+0:3]-[c:2](:[c:1]):[c:4]
null
[]
null
null
null
null
5 g of 1-(4-benzyloxy-3-hydroxymethyl-phenyl)-2-{3-[3-(4-methoxy-phenyl)-5-methyl-[1,2,4]triazol-1-yl]-1,1-dimethyl-propylamino}-ethanol dissolved in 100 mL methanol are hydrogenated under normal pressure with 1 g of palladium on charcoal (5%) as catalyst. Then the catalyst is separated off and the filtrate is evaporat...
10.6084/m9.figshare.5104873.v1
null
Ether
Aromatic alcohol
c1ccccc1
null
c1ccccc1.c1nnc[nH]1.c1ccccc1
Other
[Pd].CO
null
null
COc1ccc(-c2nc(C)n(CCC(C)(C)NCC(O)c3ccc(OCc4ccccc4)c(CO)c3)n2)cc1>[Pd].CO>COc1ccc(-c2nc(C)n(CCC(C)(C)NCC(O)c3ccc(O)c(CO)c3)n2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-0b6542bca0fa4b02977893324d8e1da7
COC(=O)c1cc(C(O)CNC(C)(C)CCN2C=CN(c3ccc(OC)cc3)C2)ccc1OCc1ccccc1>>COc1ccc(N2C=CN(CCC(C)(C)NCC(O)c3ccc(OCc4ccccc4)c(CO)c3)C2)cc1
C(C1=CC=CC=C1)OC1=C(C(=O)OC)C=C(C=C1)C(CNC(CCN1CN(C=C1)C1=CC=C(C=C1)OC)(C)C)O.[Cl-].[Ca+2].[Cl-].[BH4-].[Na+].[Cl-].[Ca+2].[Cl-].[BH4-].[Na+]>>C(C1=CC=CC=C1)OC1=C(C=C(C=C1)C(CNC(CCN1CN(C=C1)C1=CC=C(C=C1)OC)(C)C)O)CO
CO[C:33]([c:32]1[c:23]([O:24][CH2:25][c:26]2[cH:27][cH:28][cH:29][cH:30][cH:31]2)[cH:22][cH:21][c:20]([CH:18]([CH2:17][NH:16][C:13]([CH2:12][CH2:11][N:10]2[CH:9]=[CH:8][N:7]([c:6]3[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:38][cH:37]3)[CH2:36]2)([CH3:14])[CH3:15])[OH:19])[cH:35]1)=[O:34]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([N...
COC(=O)c1cc(C(O)CNC(C)(C)CCN2C=CN(c3ccc(OC)cc3)C2)ccc1OCc1ccccc1
COc1ccc(N2C=CN(CCC(C)(C)NCC(O)c3ccc(OCc4ccccc4)c(CO)c3)C2)cc1
null
null
O1CCCC1.C(C)O
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
C1=CN(c2ccccc2)CN1CCCNCCc1ccc(OCc2ccccc2)cc1
C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3](:[c:4]):[c:5]>>[OH;D1;+0:2]-[CH2;D2;+0:1]-[c:3](:[c:4]):[c:5]
null
[]
null
null
12
HOUR
13 g of methyl 2-benzyloxy-5-(1-hydroxy-2-{3-[3-(4-methoxy-phenyl)-imidazol-1-yl]-1,1-dimethyl-propylamino}-ethyl)-benzoate in 100 mL tetrahydrofuran are reacted with a solution of 6.5 g of calcium chloride in 65 mL ethanol and 4.5 g of sodium borohydride analogously to the method used for Example 1c. After a reaction ...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
c1ccccc1.C1=C[NH]C[NH]1.c1ccccc1.c1ccccc1
Other
O1CCCC1.C(C)O
null
12
COC(=O)c1cc(C(O)CNC(C)(C)CCN2C=CN(c3ccc(OC)cc3)C2)ccc1OCc1ccccc1>O1CCCC1.C(C)O>COc1ccc(N2C=CN(CCC(C)(C)NCC(O)c3ccc(OCc4ccccc4)c(CO)c3)C2)cc1
ord_dataset-c31cb9b44c404c10ba3aa533aa079e2b
ord-009ab4f6f1204a8daf3f600ee93a5576
COC(=O)c1cc(C(O)CNC(C)(C)CCn2cnc(-c3ccc(OC)cc3)n2)ccc1OCc1ccccc1>>COc1ccc(-c2ncn(CCC(C)(C)NCC(O)c3ccc(OCc4ccccc4)c(CO)c3)n2)cc1
C(C1=CC=CC=C1)OC1=C(C(=O)OC)C=C(C=C1)C(CNC(CCN1N=C(N=C1)C1=CC=C(C=C1)OC)(C)C)O.[Cl-].[Ca+2].[Cl-].[BH4-].[Na+]>>C(C1=CC=CC=C1)OC1=C(C=C(C=C1)C(CNC(CCN1N=C(N=C1)C1=CC=C(C=C1)OC)(C)C)O)CO
CO[C:33]([c:32]1[c:23]([O:24][CH2:25][c:26]2[cH:27][cH:28][cH:29][cH:30][cH:31]2)[cH:22][cH:21][c:20]([CH:18]([CH2:17][NH:16][C:13]([CH2:12][CH2:11][n:10]2[cH:9][n:8][c:7](-[c:6]3[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:38][cH:37]3)[n:36]2)([CH3:14])[CH3:15])[OH:19])[cH:35]1)=[O:34]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7...
COC(=O)c1cc(C(O)CNC(C)(C)CCn2cnc(-c3ccc(OC)cc3)n2)ccc1OCc1ccccc1
COc1ccc(-c2ncn(CCC(C)(C)NCC(O)c3ccc(OCc4ccccc4)c(CO)c3)n2)cc1
null
null
O1CCCC1.C(C)O
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
c1ccc(COc2ccc(CCNCCCn3cnc(-c4ccccc4)n3)cc2)cc1
C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3](:[c:4]):[c:5]>>[OH;D1;+0:2]-[CH2;D2;+0:1]-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
7.3 g of methyl 2-benzyloxy-5-(1-hydroxy-2-{3-[3-(4-methoxy-phenyl)-[1,2,4]triazol-1-yl]-1,1-dimethyl-propylamino}-ethyl)-benzoate are placed in 100 mL tetrahydrofuran and reduced with a total of 6.8 g of calcium chloride dissolved in ethanol and 4.6 g of sodium borohydride as described for Example 1c. The product is o...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
c1ccccc1.c1nnc[nH]1.c1ccccc1.c1ccccc1
Other
O1CCCC1.C(C)O
null
null
COC(=O)c1cc(C(O)CNC(C)(C)CCn2cnc(-c3ccc(OC)cc3)n2)ccc1OCc1ccccc1>O1CCCC1.C(C)O>COc1ccc(-c2ncn(CCC(C)(C)NCC(O)c3ccc(OCc4ccccc4)c(CO)c3)n2)cc1