dataset_id
large_stringclasses
414 values
reaction_id
large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
reactant_smiles
large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-a4cfa4d84dac4bab831418d092d51e52
O=C(OCc1ccc([N+](=O)[O-])cc1)C1=C(Oc2cccc(C(F)(F)F)c2)SC2CC(=O)N12>>O=C([O-])C1=C(Oc2cccc(C(F)(F)F)c2)SC2CC(=O)N12
O=C1CC2SC(=C(N12)C(=O)OCC1=CC=C(C=C1)[N+](=O)[O-])OC1=CC(=CC=C1)C(F)(F)F.C([O-])(O)=O.[Na+]>>O=C1CC2SC(=C(N12)C(=O)[O-])OC1=CC(=CC=C1)C(F)(F)F.[Na+]
O=[N+]([O-])c1ccc(C[O:3][C:2](=[O:1])[C:4]2=[C:5]([O:6][c:7]3[cH:8][cH:9][cH:10][c:11]([C:12]([F:13])([F:14])[F:15])[cH:16]3)[S:17][CH:18]3[CH2:19][C:20](=[O:21])[N:22]23)cc1>>[O:1]=[C:2]([O-:3])[C:4]1=[C:5]([O:6][c:7]2[cH:8][cH:9][cH:10][c:11]([C:12]([F:13])([F:14])[F:15])[cH:16]2)[S:17][CH:18]2[CH2:19][C:20](=[O:21])...
O=C(OCc1ccc([N+](=O)[O-])cc1)C1=C(Oc2cccc(C(F)(F)F)c2)SC2CC(=O)N12
O=C([O-])C1=C(Oc2cccc(C(F)(F)F)c2)SC2CC(=O)N12
null
[Pd]
O1CCOCC1.O
Miscellaneous
Ester to carboxylate
44f4ca8fa6db8bf6ed2065c1ada1557da240f35fc0d170173f2ffb8dd19aae75
572c1e76b1abdca43e2a1bb50332b6c1ee49391ecad01eed2f9507f24676fa6d
O=C1CC2SC(Oc3ccccc3)=CN12
O=[N+](-[O-])-c1:c:c:c(-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[C:4](=[C:5](-[#8:6])-[#16:7])-[#7:8]-[C:9]=[O;D1;H0:10]):c:c:1>>[#16:7]-[C:5](-[#8:6])=[C:4](-[C:2](-[O-;H0;D1:1])=[O;D1;H0:3])-[#7:8]-[C:9]=[O;D1;H0:10]
null
[]
null
null
null
null
A mixture of a solution of 602 mg of 4-nitrobenzyl 7-oxo-3-(3-trifluoromethylphenoxy)-4-thia-1-azabicyclo[3,2,0]hept-2-ene-2-carboxylate in dioxan and 108 mg sodium bicarbonate in water, and 10% palladium/charcoal was hydrogenated at 50 psi at 25° for 60 minutes. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Ester.Nitro group
null
c1ccccc1
null
c1ccccc1.C1=CN2CCC2S1
HO-
[Pd].O1CCOCC1.O
null
null
O=C(OCc1ccc([N+](=O)[O-])cc1)C1=C(Oc2cccc(C(F)(F)F)c2)SC2CC(=O)N12>[Pd].O1CCOCC1.O>O=C([O-])C1=C(Oc2cccc(C(F)(F)F)c2)SC2CC(=O)N12
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-a21876ed30be4c5880830910e25f5acc
C=CCSC1CC(=O)N1C(C(=S)OCc1ccc([N+](=O)[O-])cc1)=C(Oc1cccc2ccccc12)C(=O)C(C)(C)C.ClCl>>CC(C)(C)C(=O)C(Oc1cccc2ccccc12)=C(C(=S)OCc1ccc([N+](=O)[O-])cc1)N1C(=O)CC1Cl
C(C=C)SC1CC(N1C(C(=S)OCC1=CC=C(C=C1)[N+](=O)[O-])=C(C(C(C)(C)C)=O)OC1=CC=CC2=CC=CC=C12)=O.ClCl>>ClC1CC(N1C(C(=S)OCC1=CC=C(C=C1)[N+](=O)[O-])=C(C(C(C)(C)C)=O)OC1=CC=CC2=CC=CC=C12)=O
C=CCS[CH:37]1[N:33]([C:19](=[C:7]([C:5]([C:2]([CH3:1])([CH3:3])[CH3:4])=[O:6])[O:8][c:9]2[cH:10][cH:11][cH:12][c:13]3[cH:14][cH:15][cH:16][cH:17][c:18]23)[C:20](=[S:21])[O:22][CH2:23][c:24]2[cH:25][cH:26][c:27]([N+:28](=[O:29])[O-:30])[cH:31][cH:32]2)[C:34](=[O:35])[CH2:36]1.Cl[Cl:38]>>[CH3:1][C:2]([CH3:3])([CH3:4])[C:...
C=CCSC1CC(=O)N1C(C(=S)OCc1ccc([N+](=O)[O-])cc1)=C(Oc1cccc2ccccc12)C(=O)C(C)(C)C.ClCl
CC(C)(C)C(=O)C(Oc1cccc2ccccc12)=C(C(=S)OCc1ccc([N+](=O)[O-])cc1)N1C(=O)CC1Cl
null
null
ClCCl.C(Cl)(Cl)(Cl)Cl
Functional Group Interconversion
OtherReaction
d4a1f45948ca6338d13758a8eb064414f490d5560b79b989b8f902e12590b6c8
7fecd9068ed121180c7c8f39a016405d4e3d2c3ae4d3dd36c097f13d461df37e
O=C1CCN1C(=COc1cccc2ccccc12)C(=S)OCc1ccccc1
C=C-C-S-[CH;D3;+0:1]1-[C:2]-[C:3](=[O;D1;H0:4])-[#7:5]-1-[C:6](-[C:7](-[#8:8])=[S;D1;H0:9])=[C:10](-[#8:11])-[C:12]=[O;D1;H0:13].Cl-[Cl;H0;D1;+0:14]>>[#8:8]-[C:7](=[S;D1;H0:9])-[C:6](-[#7:5]1-[C:3](=[O;D1;H0:4])-[C:2]-[CH;D3;+0:1]-1-[Cl;H0;D1;+0:14])=[C:10](-[#8:11])-[C:12]=[O;D1;H0:13]
73.7
[{"value": 73.7, "product": "ClC1CC(N1C(C(=S)OCC1=CC=C(C=C1)[N+](=O)[O-])=C(C(C(C)(C)C)=O)OC1=CC=CC2=CC=CC=C12)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of 7.1 g of 4-nitrobenzyl 2-(4-allylthioazetidin-2-on-1-yl)-3-(1-naphthyloxy)-3-trimethylacetylthiopropenate in dichloromethane at -20° was added a solution of 23 mmol of chlorine in carbon tetrachloride. After 30 minutes the mixture was warmed to room temperature, evaporated in vacuo, and the residual oi...
10.6084/m9.figshare.5104873.v1
null
Monosulfide.Allyl
Secondary halide
C1C[NH]C1
C1C[NH]C1
c1ccc2ccccc2c1.c1ccccc1.C1C[NH]C1
HCl
ClCCl.C(Cl)(Cl)(Cl)Cl
null
null
C=CCSC1CC(=O)N1C(C(=S)OCc1ccc([N+](=O)[O-])cc1)=C(Oc1cccc2ccccc12)C(=O)C(C)(C)C.ClCl>ClCCl.C(Cl)(Cl)(Cl)Cl>CC(C)(C)C(=O)C(Oc1cccc2ccccc12)=C(C(=S)OCc1ccc([N+](=O)[O-])cc1)N1C(=O)CC1Cl
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-5f54f4ebec484876b29f0018a9c011bd
O=C(OCc1ccc([N+](=O)[O-])cc1)C1=C(Oc2cccc3ccccc23)SC2CC(=O)N12>>O=C([O-])C1=C(Oc2cccc3ccccc23)SC2CC(=O)N12
C1(=CC=CC2=CC=CC=C12)OC1=C(N2C(CC2S1)=O)C(=O)OCC1=CC=C(C=C1)[N+](=O)[O-].C([O-])(O)=O.[Na+]>>C1(=CC=CC2=CC=CC=C12)OC1=C(N2C(CC2S1)=O)C(=O)[O-].[Na+]
O=[N+]([O-])c1ccc(C[O:3][C:2](=[O:1])[C:4]2=[C:5]([O:6][c:7]3[cH:8][cH:9][cH:10][c:11]4[cH:12][cH:13][cH:14][cH:15][c:16]34)[S:17][CH:18]3[CH2:19][C:20](=[O:21])[N:22]23)cc1>>[O:1]=[C:2]([O-:3])[C:4]1=[C:5]([O:6][c:7]2[cH:8][cH:9][cH:10][c:11]3[cH:12][cH:13][cH:14][cH:15][c:16]23)[S:17][CH:18]2[CH2:19][C:20](=[O:21])[N...
O=C(OCc1ccc([N+](=O)[O-])cc1)C1=C(Oc2cccc3ccccc23)SC2CC(=O)N12
O=C([O-])C1=C(Oc2cccc3ccccc23)SC2CC(=O)N12
null
[Pd]
O1CCOCC1.O
Miscellaneous
Ester to carboxylate
44f4ca8fa6db8bf6ed2065c1ada1557da240f35fc0d170173f2ffb8dd19aae75
572c1e76b1abdca43e2a1bb50332b6c1ee49391ecad01eed2f9507f24676fa6d
O=C1CC2SC(Oc3cccc4ccccc34)=CN12
O=[N+](-[O-])-c1:c:c:c(-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[C:4](=[C:5](-[#8:6])-[#16:7])-[#7:8]-[C:9]=[O;D1;H0:10]):c:c:1>>[#16:7]-[C:5](-[#8:6])=[C:4](-[C:2](-[O-;H0;D1:1])=[O;D1;H0:3])-[#7:8]-[C:9]=[O;D1;H0:10]
null
[]
null
null
null
null
A mixture of a solution of 800 mg of 4-nitrobenzyl 3-(1-naphthyloxy)-7-oxo-4-thia-1-azabicyclo[3,2,0]hept-2-ene-2-carboxylate in dioxan and 150 mg of sodium bicarbonate in water, and 10% palladium/charcoal was hydrogenated at 50 psi at 25° for 60 minutes. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Ester.Nitro group
null
c1ccccc1
null
c1ccc2ccccc2c1.C1=CN2CCC2S1
HO-
[Pd].O1CCOCC1.O
null
null
O=C(OCc1ccc([N+](=O)[O-])cc1)C1=C(Oc2cccc3ccccc23)SC2CC(=O)N12>[Pd].O1CCOCC1.O>O=C([O-])C1=C(Oc2cccc3ccccc23)SC2CC(=O)N12
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-8bbbfe7fd6c44376ad072001ed220af4
C=CCSC1CC(=O)N1C(C(=S)OCc1ccc([N+](=O)[O-])cc1)=C(Sc1ccc(C)cc1)C(=O)C(C)(C)C.ClCl>>Cc1ccc(SC(C(=O)C(C)(C)C)=C(C(=S)OCc2ccc([N+](=O)[O-])cc2)N2C(=O)CC2Cl)cc1
C(C=C)SC1CC(N1C(C(=S)OCC1=CC=C(C=C1)[N+](=O)[O-])=C(C(C(C)(C)C)=O)SC1=CC=C(C=C1)C)=O.ClCl>>ClC1CC(N1C(C(=S)OCC1=CC=C(C=C1)[N+](=O)[O-])=C(C(C(C)(C)C)=O)SC1=CC=C(C=C1)C)=O
C=CCS[CH:32]1[N:28]([C:14](=[C:7]([S:6][c:5]2[cH:4][cH:3][c:2]([CH3:1])[cH:35][cH:34]2)[C:8](=[O:9])[C:10]([CH3:11])([CH3:12])[CH3:13])[C:15](=[S:16])[O:17][CH2:18][c:19]2[cH:20][cH:21][c:22]([N+:23](=[O:24])[O-:25])[cH:26][cH:27]2)[C:29](=[O:30])[CH2:31]1.Cl[Cl:33]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([S:6][C:7]([C:8](=[O:...
C=CCSC1CC(=O)N1C(C(=S)OCc1ccc([N+](=O)[O-])cc1)=C(Sc1ccc(C)cc1)C(=O)C(C)(C)C.ClCl
Cc1ccc(SC(C(=O)C(C)(C)C)=C(C(=S)OCc2ccc([N+](=O)[O-])cc2)N2C(=O)CC2Cl)cc1
null
null
ClCCl.C(Cl)(Cl)(Cl)Cl
Functional Group Interconversion
OtherReaction
d4a1f45948ca6338d13758a8eb064414f490d5560b79b989b8f902e12590b6c8
7fecd9068ed121180c7c8f39a016405d4e3d2c3ae4d3dd36c097f13d461df37e
O=C1CCN1C(=CSc1ccccc1)C(=S)OCc1ccccc1
C=C-C-S-[CH;D3;+0:1]1-[C:2]-[C:3](=[O;D1;H0:4])-[#7:5]-1-[C:6](-[C:7](-[#8:8])=[S;D1;H0:9])=[C:10](-[#16:11])-[C:12]=[O;D1;H0:13].Cl-[Cl;H0;D1;+0:14]>>[#16:11]-[C:10](-[C:12]=[O;D1;H0:13])=[C:6](-[#7:5]1-[C:3](=[O;D1;H0:4])-[C:2]-[CH;D3;+0:1]-1-[Cl;H0;D1;+0:14])-[C:7](-[#8:8])=[S;D1;H0:9]
69.5
[{"value": 69.5, "product": "ClC1CC(N1C(C(=S)OCC1=CC=C(C=C1)[N+](=O)[O-])=C(C(C(C)(C)C)=O)SC1=CC=C(C=C1)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of 2.28 g of 4-nitrobenzyl 2-(4-allylthioazetidin-2-on-1-yl)-3-(4-methylthiophenoxy)-3-trimethylacetylthiopropenate in dichloromethane at -20° , was added solution of 7.6 mmol of chlorine in carbon tetrachloride. After 30 minutes the mixture was warmed to room temperature, evaporated in vacuo, and the res...
10.6084/m9.figshare.5104873.v1
null
Monosulfide.Allyl
Secondary halide
C1C[NH]C1
C1C[NH]C1
c1ccccc1.c1ccccc1.C1C[NH]C1
HCl
ClCCl.C(Cl)(Cl)(Cl)Cl
null
null
C=CCSC1CC(=O)N1C(C(=S)OCc1ccc([N+](=O)[O-])cc1)=C(Sc1ccc(C)cc1)C(=O)C(C)(C)C.ClCl>ClCCl.C(Cl)(Cl)(Cl)Cl>Cc1ccc(SC(C(=O)C(C)(C)C)=C(C(=S)OCc2ccc([N+](=O)[O-])cc2)N2C(=O)CC2Cl)cc1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-708832323170435e8c8a68dfd1f9ceec
Cc1ccc(SC2=C(C(=O)OCc3ccc([N+](=O)[O-])cc3)N3C(=O)CC3S2)cc1>>Cc1ccc(SC2=C(C(=O)[O-])N3C(=O)CC3S2)cc1
CC1=CC=C(SC2=C(N3C(CC3S2)=O)C(=O)OCC2=CC=C(C=C2)[N+](=O)[O-])C=C1.C([O-])(O)=O.[Na+]>>CC1=CC=C(SC2=C(N3C(CC3S2)=O)C(=O)[O-])C=C1.[Na+]
O=[N+]([O-])c1ccc(C[O:11][C:9]([C:8]2=[C:7]([S:6][c:5]3[cH:4][cH:3][c:2]([CH3:1])[cH:19][cH:18]3)[S:17][CH:16]3[N:12]2[C:13](=[O:14])[CH2:15]3)=[O:10])cc1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([S:6][C:7]2=[C:8]([C:9](=[O:10])[O-:11])[N:12]3[C:13](=[O:14])[CH2:15][CH:16]3[S:17]2)[cH:18][cH:19]1
Cc1ccc(SC2=C(C(=O)OCc3ccc([N+](=O)[O-])cc3)N3C(=O)CC3S2)cc1
Cc1ccc(SC2=C(C(=O)[O-])N3C(=O)CC3S2)cc1
null
[Pd]
O1CCOCC1.O
Miscellaneous
Ester to carboxylate
44f4ca8fa6db8bf6ed2065c1ada1557da240f35fc0d170173f2ffb8dd19aae75
572c1e76b1abdca43e2a1bb50332b6c1ee49391ecad01eed2f9507f24676fa6d
O=C1CC2SC(Sc3ccccc3)=CN12
O=[N+](-[O-])-c1:c:c:c(-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[C:4](=[C:5](-[#16:6])-[#16:7])-[#7:8]-[C:9]=[O;D1;H0:10]):c:c:1>>[#16:7]-[C:5](-[#16:6])=[C:4](-[C:2](-[O-;H0;D1:1])=[O;D1;H0:3])-[#7:8]-[C:9]=[O;D1;H0:10]
null
[]
null
null
null
null
A mixture of a solution of 70 mg of 4-nitrobenzyl 3-(4-methylthiophenoxy)-7-oxo-4-thia-1-azabicyclo[3,2,0]hept-2-ene-2-carboxylate in dioxan and 13 mg of sodium bicarbonate in water, and 10% palladium/charcoal was hydrogenated at 50 psi at 35° for 60 minutes. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Ester.Nitro group
null
c1ccccc1
null
c1ccccc1.C1=CN2CCC2S1
HO-
[Pd].O1CCOCC1.O
null
null
Cc1ccc(SC2=C(C(=O)OCc3ccc([N+](=O)[O-])cc3)N3C(=O)CC3S2)cc1>[Pd].O1CCOCC1.O>Cc1ccc(SC2=C(C(=O)[O-])N3C(=O)CC3S2)cc1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-7c95f89235eb4b3db8041d63efaff3e4
C=CCSC1CC(=O)N1C(C(=S)OCc1ccc([N+](=O)[O-])cc1)=C(Oc1ccc(S(C)=O)cc1)C(=O)C(C)(C)C.ClCl>>CS(=O)c1ccc(OC(C(=O)C(C)(C)C)=C(C(=S)OCc2ccc([N+](=O)[O-])cc2)N2C(=O)CC2Cl)cc1
C(C=C)SC1CC(N1C(C(=S)OCC1=CC=C(C=C1)[N+](=O)[O-])=C(C(C(C)(C)C)=O)OC1=CC=C(C=C1)S(=O)C)=O.ClCl>>ClC1CC(N1C(C(=S)OCC1=CC=C(C=C1)[N+](=O)[O-])=C(C(C(C)(C)C)=O)OC1=CC=C(C=C1)S(=O)C)=O
C=CCS[CH:34]1[N:30]([C:16](=[C:9]([O:8][c:7]2[cH:6][cH:5][c:4]([S:2]([CH3:1])=[O:3])[cH:37][cH:36]2)[C:10](=[O:11])[C:12]([CH3:13])([CH3:14])[CH3:15])[C:17](=[S:18])[O:19][CH2:20][c:21]2[cH:22][cH:23][c:24]([N+:25](=[O:26])[O-:27])[cH:28][cH:29]2)[C:31](=[O:32])[CH2:33]1.Cl[Cl:35]>>[CH3:1][S:2](=[O:3])[c:4]1[cH:5][cH:6...
C=CCSC1CC(=O)N1C(C(=S)OCc1ccc([N+](=O)[O-])cc1)=C(Oc1ccc(S(C)=O)cc1)C(=O)C(C)(C)C.ClCl
CS(=O)c1ccc(OC(C(=O)C(C)(C)C)=C(C(=S)OCc2ccc([N+](=O)[O-])cc2)N2C(=O)CC2Cl)cc1
null
null
ClCCl.C(Cl)(Cl)(Cl)Cl
Functional Group Interconversion
OtherReaction
d4a1f45948ca6338d13758a8eb064414f490d5560b79b989b8f902e12590b6c8
7fecd9068ed121180c7c8f39a016405d4e3d2c3ae4d3dd36c097f13d461df37e
O=C1CCN1C(=COc1ccccc1)C(=S)OCc1ccccc1
C=C-C-S-[CH;D3;+0:1]1-[C:2]-[C:3](=[O;D1;H0:4])-[#7:5]-1-[C:6](-[C:7](-[#8:8])=[S;D1;H0:9])=[C:10](-[#8:11])-[C:12]=[O;D1;H0:13].Cl-[Cl;H0;D1;+0:14]>>[#8:8]-[C:7](=[S;D1;H0:9])-[C:6](-[#7:5]1-[C:3](=[O;D1;H0:4])-[C:2]-[CH;D3;+0:1]-1-[Cl;H0;D1;+0:14])=[C:10](-[#8:11])-[C:12]=[O;D1;H0:13]
52.5
[{"value": 52.5, "product": "ClC1CC(N1C(C(=S)OCC1=CC=C(C=C1)[N+](=O)[O-])=C(C(C(C)(C)C)=O)OC1=CC=C(C=C1)S(=O)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of 0.488 g of 4-nitrobenzyl 2-(4-allylthioazetidin-2-on-1-yl)-3-(4-methylsulphinylphenoxy)-3-trimethylacetylthiopropenate in dichloromethane at -20°, was added dropwise a solution of 1.58 mmol of chlorine in carbon tetrachloride. After 30 minutes the mixture was warmed to room temperature, evaporated in v...
10.6084/m9.figshare.5104873.v1
null
Monosulfide.Allyl
Secondary halide
C1C[NH]C1
C1C[NH]C1
c1ccccc1.c1ccccc1.C1C[NH]C1
HCl
ClCCl.C(Cl)(Cl)(Cl)Cl
null
null
C=CCSC1CC(=O)N1C(C(=S)OCc1ccc([N+](=O)[O-])cc1)=C(Oc1ccc(S(C)=O)cc1)C(=O)C(C)(C)C.ClCl>ClCCl.C(Cl)(Cl)(Cl)Cl>CS(=O)c1ccc(OC(C(=O)C(C)(C)C)=C(C(=S)OCc2ccc([N+](=O)[O-])cc2)N2C(=O)CC2Cl)cc1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-3d2edff3e0434297b73939225c1538f0
CS(=O)c1ccc(OC2=C(C(=O)OCc3ccc([N+](=O)[O-])cc3)N3C(=O)CC3S2)cc1>>CS(=O)c1ccc(OC2=C(C(=O)[O-])N3C(=O)CC3S2)cc1
CS(=O)C1=CC=C(OC2=C(N3C(CC3S2)=O)C(=O)OCC2=CC=C(C=C2)[N+](=O)[O-])C=C1.C([O-])(O)=O.[Na+]>>CS(=O)C1=CC=C(OC2=C(N3C(CC3S2)=O)C(=O)[O-])C=C1.[Na+]
O=[N+]([O-])c1ccc(C[O:13][C:11]([C:10]2=[C:9]([O:8][c:7]3[cH:6][cH:5][c:4]([S:2]([CH3:1])=[O:3])[cH:21][cH:20]3)[S:19][CH:18]3[N:14]2[C:15](=[O:16])[CH2:17]3)=[O:12])cc1>>[CH3:1][S:2](=[O:3])[c:4]1[cH:5][cH:6][c:7]([O:8][C:9]2=[C:10]([C:11](=[O:12])[O-:13])[N:14]3[C:15](=[O:16])[CH2:17][CH:18]3[S:19]2)[cH:20][cH:21]1
CS(=O)c1ccc(OC2=C(C(=O)OCc3ccc([N+](=O)[O-])cc3)N3C(=O)CC3S2)cc1
CS(=O)c1ccc(OC2=C(C(=O)[O-])N3C(=O)CC3S2)cc1
null
[Pd]
O1CCOCC1.O
Miscellaneous
Ester to carboxylate
44f4ca8fa6db8bf6ed2065c1ada1557da240f35fc0d170173f2ffb8dd19aae75
572c1e76b1abdca43e2a1bb50332b6c1ee49391ecad01eed2f9507f24676fa6d
O=C1CC2SC(Oc3ccccc3)=CN12
O=[N+](-[O-])-c1:c:c:c(-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[C:4](=[C:5](-[#8:6])-[#16:7])-[#7:8]-[C:9]=[O;D1;H0:10]):c:c:1>>[#16:7]-[C:5](-[#8:6])=[C:4](-[C:2](-[O-;H0;D1:1])=[O;D1;H0:3])-[#7:8]-[C:9]=[O;D1;H0:10]
109.8
[{"value": 109.8, "product": "CS(=O)C1=CC=C(OC2=C(N3C(CC3S2)=O)C(=O)[O-])C=C1.[Na+]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of a solution of 70 mg of 4-nitrobenzyl 3-(4-methylsulphinylphenoxy)-7-oxo-4-thia-1-azabicyclo[3,2,0]hept-2-ene-2-carboxylate in dioxan and 13 mg of sodium bicarbonate in water, and 10% palladium/charcoal was hydrogenated at 50 psi at 25° for 60 minutes. Then, the mixture was filtered through Gelite, and lyop...
10.6084/m9.figshare.5104873.v1
null
Ester.Nitro group
null
c1ccccc1
null
c1ccccc1.C1=CN2CCC2S1
HO-
[Pd].O1CCOCC1.O
null
null
CS(=O)c1ccc(OC2=C(C(=O)OCc3ccc([N+](=O)[O-])cc3)N3C(=O)CC3S2)cc1>[Pd].O1CCOCC1.O>CS(=O)c1ccc(OC2=C(C(=O)[O-])N3C(=O)CC3S2)cc1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-dc0b89bdedb5477fb9033545f5af6b61
CC(C)(C)OC(=O)CI.NC1Cc2ccccc2NC1=O>>CC(C)(C)OC(=O)CN1C(=O)C(N)Cc2ccccc21
Cl.NC1C(NC2=CC=CC=C2C1)=O.[H-].[Na+].ICC(=O)OC(C)(C)C.[H][H]>>C(C)(C)(C)OC(=O)CN1C(=O)C(CC2=CC=CC=C12)N
I[CH2:8][C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7].[NH:9]1[C:10](=[O:11])[CH:12]([NH2:13])[CH2:14][c:15]2[cH:16][cH:17][cH:18][cH:19][c:20]21>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][N:9]1[C:10](=[O:11])[CH:12]([NH2:13])[CH2:14][c:15]2[cH:16][cH:17][cH:18][cH:19][c:20]21
CC(C)(C)OC(=O)CI.NC1Cc2ccccc2NC1=O
CC(C)(C)OC(=O)CN1C(=O)C(N)Cc2ccccc21
null
null
C1CCOC1
Heteroatom Alkylation and Arylation
Boc amine protection (ethyl Boc)
00bdf42034ad419e8a7421c967f14ba303b548b011e99dd40ab321f2309531bf
933a6f1013d44497c9c5902b73c24fbdc7813d20b886bdbc4c670d5b43ca2182
O=C1CCc2ccccc2N1
I-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#8:4]-[C:5](-[C;D1;H3:6])(-[C;D1;H3:7])-[C;D1;H3:8].[C:9]-[C:10](=[O;D1;H0:11])-[NH;D2;+0:12]-[c:13](:[c:14]):[c:15]>>[C:9]-[C:10](=[O;D1;H0:11])-[N;H0;D3;+0:12](-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#8:4]-[C:5](-[C;D1;H3:6])(-[C;D1;H3:7])-[C;D1;H3:8])-[c:13](:[c:14]):[c:15]
73
[{"value": 73.0, "product": "C(C)(C)(C)OC(=O)CN1C(=O)C(CC2=CC=CC=C12)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a suspension of 2.42 gm NaH (50% oil dispersion washed 3×hexanes) in 50 ml of THF at 0° C. was added solid 5 gm (0.025 mol) of 3-aminodihydrocarbostyrilhydrochloride (T. J. McCord, Arch. of Biochem. & Biophys. 102 48 (1963)) stirring at 0° C. until the evolution of hydrogen had ceased at which time the reaction mixt...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester.Secondary amide
Ester.Tertiary amide
c1ccc2c(c1)CCCN2
c1ccc2c(c1)CCC[NH]2
c1ccc2c(c1)CCC[NH]2
HI
C1CCOC1
null
1
CC(C)(C)OC(=O)CI.NC1Cc2ccccc2NC1=O>C1CCOC1>CC(C)(C)OC(=O)CN1C(=O)C(N)Cc2ccccc21
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-68c35c50649b4a169b7dad29368e7ca8
C1=CCC2SC=CC2=C1.CC(=O)N(C)C>>CC(=O)c1cc2ccccc2s1
S1C=CC=2C1CC=CC2.[OH-].[K+].CC(=O)N(C)C.Cl>>C(C)(=O)C=1SC2=C(C1)C=CC=C2
[CH:4]1=[CH:5][C:6]2=[CH:7][CH:8]=[CH:9][CH2:10][CH:11]2[S:12]1.CN(C)[C:2]([CH3:1])=[O:3]>>[CH3:1][C:2](=[O:3])[c:4]1[cH:5][c:6]2[cH:7][cH:8][cH:9][cH:10][c:11]2[s:12]1
C1=CCC2SC=CC2=C1.CC(=O)N(C)C
CC(=O)c1cc2ccccc2s1
null
[Cu]
C(C)O
Aromatic Heterocycle Formation
OtherReaction
51f37af0025519de3472ec47d2ee9cf1eea9f404aa794312c364cac875b2133a
738ebe845e134b97f5c03ccfa6305783ef5d7282ba500cda23b85f728978db4f
c1ccc2sccc2c1
C-N(-C)-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[CH2;D2;+0:4]1-[CH;D2;+0:5]=[CH;D2;+0:6]-[CH;D2;+0:7]=[C;H0;D3;+0:8]2-[CH;D2;+0:9]=[CH;D2;+0:10]-[S;H0;D2;+0:11]-[CH;D3;+0:12]-1-2>>[C;D1;H3:2]-[C;H0;D3;+0:1](=[O;D1;H0:3])-[c;H0;D3;+0:10]1:[cH;D2;+0:9]:[c;H0;D3;+0:8]2:[cH;D2;+0:7]:[cH;D2;+0:6]:[cH;D2;+0:5]:[cH;D2;+0:4]:...
70
[{"value": 70.0, "product": "C(C)(=O)C=1SC2=C(C1)C=CC=C2", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The amino ester (2) was converted to the diazonium salt and reduced by boiling in ethanol containing finely divided copper to give the pure ester (3). Hydrolysis of the ester with aqueous ethanolic KOH followed by acidification with 5M HCl, gave the acid (4) in approximately 70% yield. The acid was converted to the cor...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Monosulfide.Conjugated diene
Ketone
C1=CCC2SC=CC2=C1
c1ccc2sccc2c1
c1ccc2sccc2c1
Other
[Cu].C(C)O
null
null
C1=CCC2SC=CC2=C1.CC(=O)N(C)C>[Cu].C(C)O>CC(=O)c1cc2ccccc2s1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-4fc6a07ca93446d38317ff7a8bd2f484
C=C(Cl)C#N.NNc1ccccc1>>Nc1ccnn1-c1ccccc1
[OH-].[Na+].C1(=CC=CC=C1)NN.ClC(C#N)=C>>C1(=CC=CC=C1)N1N=CC=C1N
Cl[C:3]([C:2]#[N:1])=[CH2:4].[NH2:5][NH:6][c:7]1[cH:8][cH:9][cH:10][cH:11][cH:12]1>>[NH2:1][c:2]1[cH:3][cH:4][n:5][n:6]1-[c:7]1[cH:8][cH:9][cH:10][cH:11][cH:12]1
C=C(Cl)C#N.NNc1ccccc1
Nc1ccnn1-c1ccccc1
null
null
O
Aromatic Heterocycle Formation
OtherReaction
73db7ff77744011e446624a12a8f2967f91e152d48aa4b0429cb6519236bbd1a
0ef1207b247725ba3e9988175e67d1a1cbc24b547bfa121f8d76996eaac432f4
c1ccc(-n2cccn2)cc1
Cl-[C;H0;D3;+0:1](=[CH2;D1;+0:2])-[C;H0;D2;+0:3]#[N;H0;D1;+0:4].[NH2;D1;+0:5]-[NH;D2;+0:6]-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10]:[c:11]>>[NH2;D1;+0:4]-[c;H0;D3;+0:3]1:[cH;D2;+0:1]:[cH;D2;+0:2]:[n;H0;D2;+0:5]:[n;H0;D3;+0:6]:1-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10]:[c:11]
null
[]
null
null
6
HOUR
To a mixture consisting of 680 parts water, 216 parts of phenylhydrazine and 164 parts of 2-chloroacrylonitrile 220 parts of a 30% sodium hydroxide solution are added dropwise at room temperature. After six hours the reaction is completed. The resulting 1-phenyl-5-aminopyrazole is isolated from that phase which has bee...
10.6084/m9.figshare.5104873.v1
null
Hydrazine.Alkenyl halide.Nitrile.Vinyl
Primary amine
null
c1cc[nH]n1
c1cc[nH]n1.c1ccccc1
HCl
O
null
6
C=C(Cl)C#N.NNc1ccccc1>O>Nc1ccnn1-c1ccccc1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-7bca2b98e81b4d6c8d6a97745045e45b
O=C(O)c1cc(Oc2ccc(C(F)(F)F)cc2Cl)ccc1[N+](=O)[O-].O=S(Cl)Cl>>O=C(Cl)c1cc(Oc2ccc(C(F)(F)F)cc2Cl)ccc1[N+](=O)[O-]
[N+](=O)([O-])C1=C(C(=O)O)C=C(C=C1)OC1=C(C=C(C=C1)C(F)(F)F)Cl.S(=O)(Cl)Cl>>[N+](=O)([O-])C1=C(C(=O)Cl)C=C(C=C1)OC1=C(C=C(C=C1)C(F)(F)F)Cl
O[C:2](=[O:1])[c:4]1[cH:5][c:6]([O:7][c:8]2[cH:9][cH:10][c:11]([C:12]([F:13])([F:14])[F:15])[cH:16][c:17]2[Cl:18])[cH:19][cH:20][c:21]1[N+:22](=[O:23])[O-:24].O=S(Cl)[Cl:3]>>[O:1]=[C:2]([Cl:3])[c:4]1[cH:5][c:6]([O:7][c:8]2[cH:9][cH:10][c:11]([C:12]([F:13])([F:14])[F:15])[cH:16][c:17]2[Cl:18])[cH:19][cH:20][c:21]1[N+:22...
O=C(O)c1cc(Oc2ccc(C(F)(F)F)cc2Cl)ccc1[N+](=O)[O-].O=S(Cl)Cl
O=C(Cl)c1cc(Oc2ccc(C(F)(F)F)cc2Cl)ccc1[N+](=O)[O-]
null
null
null
Functional Group Interconversion
Alcohol to chloride_SOCl2
c301c14a9dcd0670d52e8b77396cbe7fd8edeedd757bc43f4162ade1fc52fc93
787f545db5dc0b29dde55b5fbed7db8625b8055f49327f97ed4d83cc47c3af1d
c1ccc(Oc2ccccc2)cc1
Cl-S(=O)-[Cl;H0;D1;+0:1].O-[C;H0;D3;+0:2](=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]>>[Cl;H0;D1;+0:1]-[C;H0;D3;+0:2](=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]
null
[]
null
null
null
null
0.3 Part of 2-nitro-5-(2-chloro-4-trifluoromethylphenoxy)benzoic acid and 0.83 part of thionyl chloride for 2 hours. After the reaction, the excess of thionyl chloride was removed under reduced pressure to give 0.31 part of 2-nitro-5-(2-chloro-4-trifluoromethylphenoxy)benzoyl chloride. The resulting benzoyl chloride wa...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Acyl halide
null
null
c1ccccc1.c1ccccc1
HCl
null
null
null
O=C(O)c1cc(Oc2ccc(C(F)(F)F)cc2Cl)ccc1[N+](=O)[O-].O=S(Cl)Cl>>O=C(Cl)c1cc(Oc2ccc(C(F)(F)F)cc2Cl)ccc1[N+](=O)[O-]
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-43deab324a3240d394a7343e641e646e
CC(Oc1ccc(Oc2ccc(C(F)(F)F)cn2)cc1)C(=O)Cl.CCCCCCCCCCCCO>>CCCCCCCCCCCCOC(=O)C(C)Oc1ccc(Oc2ccc(C(F)(F)F)cn2)cc1
FC(C=1C=CC(=NC1)OC1=CC=C(OC(C(=O)Cl)C)C=C1)(F)F.C(CCCCCCCCCCC)O.C(C)N(CC)CC>>FC(C=1C=CC(=NC1)OC1=CC=C(OC(C(=O)OCCCCCCCCCCCC)C)C=C1)(F)F
Cl[C:14](=[O:15])[CH:16]([CH3:17])[O:18][c:19]1[cH:20][cH:21][c:22]([O:23][c:24]2[cH:25][cH:26][c:27]([C:28]([F:29])([F:30])[F:31])[cH:32][n:33]2)[cH:34][cH:35]1.[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][OH:13]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH2:9...
CC(Oc1ccc(Oc2ccc(C(F)(F)F)cn2)cc1)C(=O)Cl.CCCCCCCCCCCCO
CCCCCCCCCCCCOC(=O)C(C)Oc1ccc(Oc2ccc(C(F)(F)F)cn2)cc1
null
null
C1(=CC=CC=C1)C
Acylation
Schotten-Baumann to ester
6cefe709828c5bd4655f254e75d5dff9e8876e192e7dd47256c1bc0067bc5291
d8a7643b81ed07a6f633aa99465180dfa0565e61ae25aef36338ebb9837c9cef
c1ccc(Oc2ccccn2)cc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[#8:4])-[C;D1;H3:5].[C:6]-[C:7]-[OH;D1;+0:8]>>[#8:4]-[C:3](-[C;D1;H3:5])-[C;H0;D3;+0:1](=[O;D1;H0:2])-[O;H0;D2;+0:8]-[C:7]-[C:6]
null
[]
10
CELSIUS
null
null
n-Dodecanol(2.5 grams; 0.134mol), toluene (80 ml) and triethylamine (5 ml) were placed into a 300 ml, 3-necked glass reaction flask equipped with stirrer, thermometer, reflux condenser, and nitrogen line. 2-[4-(5-trifluoromethyl-2-pyridinyloxy)phenoxy]propanoic acid chloride (4.45 grams; 0.0125 mol) in toluene (30 ml) ...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary alcohol
Ester
null
null
c1ccccc1.c1ccncc1
HCl
C1(=CC=CC=C1)C
10
null
CC(Oc1ccc(Oc2ccc(C(F)(F)F)cn2)cc1)C(=O)Cl.CCCCCCCCCCCCO>C1(=CC=CC=C1)C>CCCCCCCCCCCCOC(=O)C(C)Oc1ccc(Oc2ccc(C(F)(F)F)cn2)cc1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-f55734ffe0484999bc43846da7949556
Clc1cccc(C(Oc2ccccc2)Oc2ccccc2)n1>>c1ccc(OC(Oc2ccccc2)c2ccccn2)cc1
ClC1=CC=CC(=N1)C(OC1=CC=CC=C1)OC1=CC=CC=C1.C(C)N(CC)CC.[H][H]>>O(C1=CC=CC=C1)C(C1=NC=CC=C1)OC1=CC=CC=C1
Cl[c:18]1[cH:17][cH:16][cH:15][c:14]([CH:6]([O:5][c:4]2[cH:3][cH:2][cH:1][cH:21][cH:20]2)[O:7][c:8]2[cH:9][cH:10][cH:11][cH:12][cH:13]2)[n:19]1>>[cH:1]1[cH:2][cH:3][c:4]([O:5][CH:6]([O:7][c:8]2[cH:9][cH:10][cH:11][cH:12][cH:13]2)[c:14]2[cH:15][cH:16][cH:17][cH:18][n:19]2)[cH:20][cH:21]1
Clc1cccc(C(Oc2ccccc2)Oc2ccccc2)n1
c1ccc(OC(Oc2ccccc2)c2ccccn2)cc1
null
[Pd]
C(C)O
Functional Group Interconversion
Aromatic dehalogenation
ea85ec2fde5700c76b45764563e70d433b50e38e1af4209f646f155266c8ec96
56de34d4a44cb25d9380269ee5e138b0f24b40a3a0db22c5508049dc775a861f
c1ccc(OC(Oc2ccccc2)c2ccccn2)cc1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5]>>[c:3]:[#7;a:2]:[cH;D2;+0:1]:[c:4]:[c:5]
null
[]
null
null
null
null
To a solution of 10.42 grams (g) (0.032 mole (m)) of 6-chloro-2-(diphenoxy-methyl)pyridine, 8.02 g (0.079 m) of triethylamine in 200 milliliters (ml) of absolute ethanol in a Parr shaker bottle was added 0.5 g of 5 percent palladium on charcoal. Hydrogen was passed over the liquid surface using a Parr hydrogenator unti...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1ccncc1
c1ccncc1
c1ccccc1.c1ccccc1.c1ccncc1
Other
[Pd].C(C)O
null
null
Clc1cccc(C(Oc2ccccc2)Oc2ccccc2)n1>[Pd].C(C)O>c1ccc(OC(Oc2ccccc2)c2ccccn2)cc1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-b5500c318dd6471eb5ce61af6b4af19b
CCO.Clc1cccc(C(Oc2ccccc2)Oc2ccccc2)n1>>CCOc1cccc(C(Oc2ccccc2)Oc2ccccc2)n1
[H][H].[Na].C(C)O.[Na].ClC1=CC=CC(=N1)C(OC1=CC=CC=C1)OC1=CC=CC=C1>>C(C)OC1=CC=CC(=N1)C(OC1=CC=CC=C1)OC1=CC=CC=C1
[CH3:1][CH2:2][OH:3].Cl[c:4]1[cH:5][cH:6][cH:7][c:8]([CH:9]([O:10][c:11]2[cH:12][cH:13][cH:14][cH:15][cH:16]2)[O:17][c:18]2[cH:19][cH:20][cH:21][cH:22][cH:23]2)[n:24]1>>[CH3:1][CH2:2][O:3][c:4]1[cH:5][cH:6][cH:7][c:8]([CH:9]([O:10][c:11]2[cH:12][cH:13][cH:14][cH:15][cH:16]2)[O:17][c:18]2[cH:19][cH:20][cH:21][cH:22][cH:...
CCO.Clc1cccc(C(Oc2ccccc2)Oc2ccccc2)n1
CCOc1cccc(C(Oc2ccccc2)Oc2ccccc2)n1
null
null
O.CS(=O)C
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
ea617b323b892eda23f5ae30e789991ea9692064ef355a16e8ed81c16e743d2b
a4cafa7bcd156e21cca6eaac1b32e28ec8540642a31181122e6957f3d7559631
c1ccc(OC(Oc2ccccc2)c2ccccn2)cc1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5].[C;D1;H3:6]-[C:7]-[OH;D1;+0:8]>>[C;D1;H3:6]-[C:7]-[O;H0;D2;+0:8]-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5]
null
[]
80
CELSIUS
24
HOUR
To 30.0 ml of ethanol was added 1.10 g of sodium pellets. After the sodium had dissolved, 10.14 g of 6-chloro-2-(diphenoxymethyl)pyridine in 50 ml of DMSO was added dropwise. The mixture was heated to 80° C. and held there for 24 hours. The reaction was considered complete as seen by the NMR. The reaction mixture was c...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary alcohol
Ether
c1ccncc1
c1ccncc1
c1ccncc1.c1ccccc1.c1ccccc1
HCl
O.CS(=O)C
80
24
CCO.Clc1cccc(C(Oc2ccccc2)Oc2ccccc2)n1>O.CS(=O)C>CCOc1cccc(C(Oc2ccccc2)Oc2ccccc2)n1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-1c364b92de084a02a850268fe3d787b6
CS.Clc1cccc(C(Oc2ccccc2)Oc2ccccc2)n1>>CSc1cccc(C(Oc2ccccc2)Oc2ccccc2)n1
ClC1=CC=CC(=N1)C(OC1=CC=CC=C1)OC1=CC=CC=C1.C[O-].[Na+].[Na].CS>>CSC1=CC=CC(=N1)C(OC1=CC=CC=C1)OC1=CC=CC=C1
[CH3:1][SH:2].Cl[c:3]1[cH:4][cH:5][cH:6][c:7]([CH:8]([O:9][c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[O:16][c:17]2[cH:18][cH:19][cH:20][cH:21][cH:22]2)[n:23]1>>[CH3:1][S:2][c:3]1[cH:4][cH:5][cH:6][c:7]([CH:8]([O:9][c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[O:16][c:17]2[cH:18][cH:19][cH:20][cH:21][cH:22]2)[n:23]1
CS.Clc1cccc(C(Oc2ccccc2)Oc2ccccc2)n1
CSc1cccc(C(Oc2ccccc2)Oc2ccccc2)n1
null
null
CS(=O)C.CO
Heteroatom Alkylation and Arylation
Ullmann-Goldberg Substitution thiol
83e1471f87e837809a4e2fb3e1de305c0d7a6603480e04a86024c7cd55ed85fb
b7fe376f7aad2517725eef26ab981e4baa6c31c5f38fdf89e7c52a4a2c6cc1d2
c1ccc(OC(Oc2ccccc2)c2ccccn2)cc1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5].[C;D1;H3:6]-[SH;D1;+0:7]>>[C;D1;H3:6]-[S;H0;D2;+0:7]-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5]
null
[]
13
CELSIUS
null
null
To a mixture of sodium methoxide (made from 100 ml (2.47 m) of methanol and 1.50 g (0.652 m) of sodium metal) which had been cooled to 13° C. was added 7.0 ml (0.126 m) of methylmercaptan. The mixture was allowed to warm to room temperature and then 20.0 g of 6-chloro-2-(diphenoxymethyl)pyridine and 150 ml of dimethyls...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aliphatic thiol
Monosulfide
c1ccncc1
c1ccncc1
c1ccncc1.c1ccccc1.c1ccccc1
HCl
CS(=O)C.CO
13
null
CS.Clc1cccc(C(Oc2ccccc2)Oc2ccccc2)n1>CS(=O)C.CO>CSc1cccc(C(Oc2ccccc2)Oc2ccccc2)n1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-d502269df27c49a786d313339978d5bd
CSC(=NC#N)SC.NS(=O)(=O)c1ccccc1[N+](=O)[O-]>>CSC(=NC#N)NS(=O)(=O)c1ccccc1[N+](=O)[O-]
[N+](=O)([O-])C1=C(C=CC=C1)S(=O)(=O)N.CSC(=NC#N)SC.C(=O)([O-])[O-].[K+].[K+]>>C(#N)N=C(NS(=O)(=O)C1=C(C=CC=C1)[N+](=O)[O-])SC
CS[C:3]([S:2][CH3:1])=[N:4][C:5]#[N:6].[NH2:7][S:8](=[O:9])(=[O:10])[c:11]1[cH:12][cH:13][cH:14][cH:15][c:16]1[N+:17](=[O:18])[O-:19]>>[CH3:1][S:2][C:3](=[N:4][C:5]#[N:6])[NH:7][S:8](=[O:9])(=[O:10])[c:11]1[cH:12][cH:13][cH:14][cH:15][c:16]1[N+:17](=[O:18])[O-:19]
CSC(=NC#N)SC.NS(=O)(=O)c1ccccc1[N+](=O)[O-]
CSC(=NC#N)NS(=O)(=O)c1ccccc1[N+](=O)[O-]
null
null
CC(=O)C
Heteroatom Alkylation and Arylation
OtherReaction
ba95383ce51db2717e65e6a878156c5ff7d731f3f5512dc0487b6cd8ce3c344d
113461c1621d86500c6bddb99471970dcbe90dcd3b57be697f00b24c57c3b50f
c1ccccc1
C-S-[C;H0;D3;+0:1](-[#16:2]-[C;D1;H3:3])=[#7:4]-[C:5]#[N;D1;H0:6].[NH2;D1;+0:7]-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11]>>[C;D1;H3:3]-[#16:2]-[C;H0;D3;+0:1](=[#7:4]-[C:5]#[N;D1;H0:6])-[NH;D2;+0:7]-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11]
55
[{"value": 55.0, "product": "C(#N)N=C(NS(=O)(=O)C1=C(C=CC=C1)[N+](=O)[O-])SC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 54.9, "product": "C(#N)N=C(NS(=O)(=O)C1=C(C=CC=C1)[N+](=O)[O-])SC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
A mixture of 2.02 g (10.0 mmol) of 2-nitrobenzene-sulfonamide, 1.46 g (10.0 mmol) of dimethyl N-cyanodithioiminocarbonate and 1.38 g (10.0 mmol) of powdered, anydrous K2CO3 in 16 ml of acetone was heated at reflux for 20 hours. The reaction mixture was filtered and the solid collected was washed several times with acet...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Monosulfide.Monosulfide
Sulfonamide.Monosulfide
null
null
c1ccccc1
Other
CC(=O)C
null
1
CSC(=NC#N)SC.NS(=O)(=O)c1ccccc1[N+](=O)[O-]>CC(=O)C>CSC(=NC#N)NS(=O)(=O)c1ccccc1[N+](=O)[O-]
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-1be0027e2f07480ca70d4b072b028c1d
CSC(=NC#N)NS(=O)(=O)c1ccccc1[N+](=O)[O-].NN>>Nc1nc(NS(=O)(=O)c2ccccc2[N+](=O)[O-])n[nH]1
C(#N)N=C(NS(=O)(=O)C1=C(C=CC=C1)[N+](=O)[O-])SC.NN>>NC1=NC(=NN1)NS(=O)(=O)C1=C(C=CC=C1)[N+](=O)[O-]
CS[C:4](=[N:3][C:2]#[N:1])[NH:5][S:6](=[O:7])(=[O:8])[c:9]1[cH:10][cH:11][cH:12][cH:13][c:14]1[N+:15](=[O:16])[O-:17].[NH2:18][NH2:19]>>[NH2:1][c:2]1[n:3][c:4]([NH:5][S:6](=[O:7])(=[O:8])[c:9]2[cH:10][cH:11][cH:12][cH:13][c:14]2[N+:15](=[O:16])[O-:17])[n:18][nH:19]1
CSC(=NC#N)NS(=O)(=O)c1ccccc1[N+](=O)[O-].NN
Nc1nc(NS(=O)(=O)c2ccccc2[N+](=O)[O-])n[nH]1
null
null
C(C)#N
Aromatic Heterocycle Formation
OtherReaction
4334099462ff9bb73d9e35682bf6cbb1a8632d3da77de0bc558fc71a8eb2c1bd
846c6feeda9d596d616e97acabee3af65330745e99fec7539883dfed54df91fa
O=S(=O)(Nc1nc[nH]n1)c1ccccc1
C-S-[C;H0;D3;+0:1](-[#7:2]-[#16:3])=[N;H0;D2;+0:4]-[C;H0;D2;+0:5]#[N;H0;D1;+0:6].[NH2;D1;+0:7]-[NH2;D1;+0:8]>>[#16:3]-[#7:2]-[c;H0;D3;+0:1]1:[n;H0;D2;+0:7]:[nH;D2;+0:8]:[c;H0;D3;+0:5](-[NH2;D1;+0:6]):[n;H0;D2;+0:4]:1
82.2
[{"value": 82.2, "product": "NC1=NC(=NN1)NS(=O)(=O)C1=C(C=CC=C1)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
9
DAY
A suspension of 29.4 g (98.0 mmol) of N'-Cyano-N-(2-nitrophenylsulfonyl)-S-methylisothiourea in 100 ml of acetonitrile was treated with 6.2 ml (6.3 g, 0.20 mol) of anhydrous hydrazine. A mild exothermic reaction occurred as the reaction mixture became homogeneous. After stirring for 9 days the precipitated solid was co...
10.6084/m9.figshare.5104873.v1
null
Hydrazine.Nitrile.Monosulfide
Primary amine
null
c1nnc[nH]1
c1nnc[nH]1.c1ccccc1
Other
C(C)#N
null
216
CSC(=NC#N)NS(=O)(=O)c1ccccc1[N+](=O)[O-].NN>C(C)#N>Nc1nc(NS(=O)(=O)c2ccccc2[N+](=O)[O-])n[nH]1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-12c44bf2a720460bb09bece297db259d
CSC(=NC#N)SC.NS(=O)(=O)c1cc(Cl)ccc1Cl>>CSC(=NC#N)NS(=O)(=O)c1cc(Cl)ccc1Cl
ClC1=C(C=C(C=C1)Cl)S(=O)(=O)N.CSC(=NC#N)SC.[OH-].[Na+].Cl>>C(#N)N=C(NS(=O)(=O)C1=C(C=CC(=C1)Cl)Cl)SC
CS[C:3]([S:2][CH3:1])=[N:4][C:5]#[N:6].[NH2:7][S:8](=[O:9])(=[O:10])[c:11]1[cH:12][c:13]([Cl:14])[cH:15][cH:16][c:17]1[Cl:18]>>[CH3:1][S:2][C:3](=[N:4][C:5]#[N:6])[NH:7][S:8](=[O:9])(=[O:10])[c:11]1[cH:12][c:13]([Cl:14])[cH:15][cH:16][c:17]1[Cl:18]
CSC(=NC#N)SC.NS(=O)(=O)c1cc(Cl)ccc1Cl
CSC(=NC#N)NS(=O)(=O)c1cc(Cl)ccc1Cl
null
null
O.C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
ba95383ce51db2717e65e6a878156c5ff7d731f3f5512dc0487b6cd8ce3c344d
113461c1621d86500c6bddb99471970dcbe90dcd3b57be697f00b24c57c3b50f
c1ccccc1
C-S-[C;H0;D3;+0:1](-[#16:2]-[C;D1;H3:3])=[#7:4]-[C:5]#[N;D1;H0:6].[NH2;D1;+0:7]-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11]>>[C;D1;H3:3]-[#16:2]-[C;H0;D3;+0:1](=[#7:4]-[C:5]#[N;D1;H0:6])-[NH;D2;+0:7]-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11]
60.7
[{"value": 60.7, "product": "C(#N)N=C(NS(=O)(=O)C1=C(C=CC(=C1)Cl)Cl)SC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 10.6 g (43.2 mmol) of 2,5-dichlorobenzenesulfonamide, 7.15 g (44.0 mmol) of 90 percent dimethyl N-cyanodithioiminocarbonate and 1.8 g (44 mmol) of NaOH in 60 ml of ethanol and 10 ml of H2O was heated at reflux for 6 hours. After cooling to room temperature the reaction mixture was poured into 600 ml of ic...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Monosulfide.Monosulfide
Sulfonamide.Monosulfide
null
null
c1ccccc1
Other
O.C(C)O
null
null
CSC(=NC#N)SC.NS(=O)(=O)c1cc(Cl)ccc1Cl>O.C(C)O>CSC(=NC#N)NS(=O)(=O)c1cc(Cl)ccc1Cl
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-6342821919ea4f479e4c2717e781a086
CSC(=NC#N)NS(=O)(=O)c1cc(Cl)ccc1Cl.NN>>Nc1nc(NS(=O)(=O)c2cc(Cl)ccc2Cl)n[nH]1
C(#N)N=C(NS(=O)(=O)C1=C(C=CC(=C1)Cl)Cl)SC.O.NN>>NC1=NC(=NN1)NS(=O)(=O)C1=C(C=CC(=C1)Cl)Cl
CS[C:4](=[N:3][C:2]#[N:1])[NH:5][S:6](=[O:7])(=[O:8])[c:9]1[cH:10][c:11]([Cl:12])[cH:13][cH:14][c:15]1[Cl:16].[NH2:17][NH2:18]>>[NH2:1][c:2]1[n:3][c:4]([NH:5][S:6](=[O:7])(=[O:8])[c:9]2[cH:10][c:11]([Cl:12])[cH:13][cH:14][c:15]2[Cl:16])[n:17][nH:18]1
CSC(=NC#N)NS(=O)(=O)c1cc(Cl)ccc1Cl.NN
Nc1nc(NS(=O)(=O)c2cc(Cl)ccc2Cl)n[nH]1
null
null
C(C)O
Aromatic Heterocycle Formation
OtherReaction
4334099462ff9bb73d9e35682bf6cbb1a8632d3da77de0bc558fc71a8eb2c1bd
846c6feeda9d596d616e97acabee3af65330745e99fec7539883dfed54df91fa
O=S(=O)(Nc1nc[nH]n1)c1ccccc1
C-S-[C;H0;D3;+0:1](-[#7:2]-[#16:3])=[N;H0;D2;+0:4]-[C;H0;D2;+0:5]#[N;H0;D1;+0:6].[NH2;D1;+0:7]-[NH2;D1;+0:8]>>[#16:3]-[#7:2]-[c;H0;D3;+0:1]1:[n;H0;D2;+0:7]:[nH;D2;+0:8]:[c;H0;D3;+0:5](-[NH2;D1;+0:6]):[n;H0;D2;+0:4]:1
63.2
[{"value": 57.0, "product": "NC1=NC(=NN1)NS(=O)(=O)C1=C(C=CC(=C1)Cl)Cl", "details": "PERCENTYIELD", "is_desired": false}, {"value": 63.2, "product": "NC1=NC(=NN1)NS(=O)(=O)C1=C(C=CC(=C1)Cl)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
A mixture of 8.51 g (26.2 mmol) of N'-cyano-N-(2,5-dichlorophenylsulfonyl)-S-methylisothiourea and 10 ml (10 g, 0.20 mol) of hydrazine monohydrate in 85 ml of ethanol was heated at reflux for 30 minutes. After cooling to room temperature, the solid which separated was collected and suspended in 170 ml of H2O and the su...
10.6084/m9.figshare.5104873.v1
null
Hydrazine.Nitrile.Monosulfide
Primary amine
null
c1nnc[nH]1
c1nnc[nH]1.c1ccccc1
Other
C(C)O
null
4
CSC(=NC#N)NS(=O)(=O)c1cc(Cl)ccc1Cl.NN>C(C)O>Nc1nc(NS(=O)(=O)c2cc(Cl)ccc2Cl)n[nH]1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-a3f93e06bdb3443090fa16797409ab1b
CC(=O)Cl.CCOC(C)=N>>CCOC(C)=NC(C)=O
CCOCC.C(C)N(CC)CC.Cl.C(C)(OCC)=N.C(C)(=O)Cl>>C(C)(=O)N=C(C)OCC
Cl[C:7]([CH3:8])=[O:9].[CH3:1][CH2:2][O:3][C:4]([CH3:5])=[NH:6]>>[CH3:1][CH2:2][O:3][C:4]([CH3:5])=[N:6][C:7]([CH3:8])=[O:9]
CC(=O)Cl.CCOC(C)=N
CCOC(C)=NC(C)=O
null
null
C(Cl)Cl
Acylation
OtherReaction
179ae8baa325b2dace7c965a68a4b2b7e91bea49291f7cdbcd29e5947f465078
edbcca52d877d662e04f0d6de1a7107a8eca1d366ee6da0d92e37eb02a291876
null
Cl-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[#8:4]-[C:5](-[C;D1;H3:6])=[NH;D1;+0:7]>>[#8:4]-[C:5](-[C;D1;H3:6])=[N;H0;D2;+0:7]-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3]
null
[]
null
null
1
HOUR
A slurry of 50.0 gm (405 mmol) of ethyl acetimidate hydrochloride in 500 ml of methylene chloride was mechanically stirred and treated dropwise with 81.9 gm (809 mmol) of triethylamine while keeping the temperature at less than 25° C. The resulting slurry was then treated dropwise with 31.8 gm (405 mmol) of acetyl chlo...
10.6084/m9.figshare.5104873.v1
null
Acyl halide
null
null
null
null
HCl
C(Cl)Cl
null
1
CC(=O)Cl.CCOC(C)=N>C(Cl)Cl>CCOC(C)=NC(C)=O
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-3873046c49ec48d7830f08215588ea91
C=O.COc1cc(C)nc(N)n1.Sc1ccc(Cl)cc1>>COc1cc(C)nc(NCSc2ccc(Cl)cc2)n1
NC1=NC(=CC(=N1)OC)C.ClC1=CC=C(C=C1)S.C=O.C(C)(=O)O>>ClC1=CC=C(C=C1)SCNC1=NC(=CC(=N1)OC)C
O=[CH2:10].[CH3:1][O:2][c:3]1[cH:4][c:5]([CH3:6])[n:7][c:8]([NH2:9])[n:19]1.[SH:11][c:12]1[cH:13][cH:14][c:15]([Cl:16])[cH:17][cH:18]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]([CH3:6])[n:7][c:8]([NH:9][CH2:10][S:11][c:12]2[cH:13][cH:14][c:15]([Cl:16])[cH:17][cH:18]2)[n:19]1
C=O.COc1cc(C)nc(N)n1.Sc1ccc(Cl)cc1
COc1cc(C)nc(NCSc2ccc(Cl)cc2)n1
null
null
CO
Heteroatom Alkylation and Arylation
OtherReaction
2d0fe4ff000088d00236210328e6740a8e7263313cbd40d392304d162b9c89b9
6e2397efe34d7315a5ce483455c7df26531092f417dbaca10e4c007fcfdb0f77
c1ccc(SCNc2ncccn2)cc1
O=[CH2;D1;+0:1].[NH2;D1;+0:2]-[c:3](:[#7;a:4]:[c:5]):[#7;a:6]:[c:7].[SH;D1;+0:8]-[c:9](:[c:10]):[c:11]>>[c:10]:[c:9](-[S;H0;D2;+0:8]-[CH2;D2;+0:1]-[NH;D2;+0:2]-[c:3](:[#7;a:4]:[c:5]):[#7;a:6]:[c:7]):[c:11]
null
[]
null
null
null
null
A mixture of 13.99 g of 2-amino-4-methoxy-6-methylpyrimidine (0.1 mole), 14.8 g of 4-chlorothiophenol (0.1 mole), 9.4 g of aqueous 35% formaldehyde (0.11 mole) and 1 g of acetic acid are heated under reflux for 1 hour in 100 ml of methanol. The resultant solution is clarified by filtration, diluted with 150 ml of tolue...
10.6084/m9.figshare.5104873.v1
null
Formaldehyde.Primary amine.Aromatic thiol
Secondary amine.Monosulfide
null
null
c1cncnc1.c1ccccc1
HO-
CO
null
null
C=O.COc1cc(C)nc(N)n1.Sc1ccc(Cl)cc1>CO>COc1cc(C)nc(NCSc2ccc(Cl)cc2)n1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-6791810aca4f480999d23281a8ce7cc3
C=O.COc1nc(N)nc(N(C)C)n1.Cc1ccc(S(=O)O)cc1>>COc1nc(NCS(=O)(=O)c2ccc(C)cc2)nc(N(C)C)n1
NC1=NC(=NC(=N1)N(C)C)OC.C1(=CC=C(C=C1)S(=O)O)C.CS(=O)(=O)O.C=O.[Na]>>CN(C1=NC(=NC(=N1)OC)NCS(=O)(=O)C1=CC=C(C=C1)C)C
O=[CH2:7].[CH3:1][O:2][c:3]1[n:4][c:5]([NH2:6])[n:18][c:19]([N:20]([CH3:21])[CH3:22])[n:23]1.[S:8]([OH:9])(=[O:10])[c:11]1[cH:12][cH:13][c:14]([CH3:15])[cH:16][cH:17]1>>[CH3:1][O:2][c:3]1[n:4][c:5]([NH:6][CH2:7][S:8](=[O:9])(=[O:10])[c:11]2[cH:12][cH:13][c:14]([CH3:15])[cH:16][cH:17]2)[n:18][c:19]([N:20]([CH3:21])[CH3:...
C=O.COc1nc(N)nc(N(C)C)n1.Cc1ccc(S(=O)O)cc1
COc1nc(NCS(=O)(=O)c2ccc(C)cc2)nc(N(C)C)n1
null
null
O.CO
Oxidation
OtherReaction
4c8dd97d415b48657455bb0302975e9329dde32a651672aa651ffaf78b0a7de9
52176cde990f5626106e5ae726067cfff0928faa899ed213a94af53862fdf1d0
O=S(=O)(CNc1ncncn1)c1ccccc1
O=[CH2;D1;+0:1].[NH2;D1;+0:2]-[c:3]1:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:[#7;a:8]:1.[O;D1;H0:9]=[S;H0;D3;+0:10](-[OH;D1;+0:11])-[c:12](:[c:13]):[c:14]>>[O;D1;H0:9]=[S;H0;D4;+0:10](=[O;H0;D1;+0:11])(-[CH2;D2;+0:1]-[NH;D2;+0:2]-[c:3]1:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:[#7;a:8]:1)-[c:12](:[c:13]):[c:14]
null
[]
null
null
30
MINUTE
8.5 g (0.05 mole) of 2-amino-4-dimethylamino-6-methoxy-1,3,5-triazine and 9.1 g (0.05 mole) of toluene-4-sulfinic acid, sodium salt, are suspended in 100 ml of methanol and to the stirred suspension are added, in succession, 4.8 g (0.05 mole) of methanesulfonic acid and 4.7 g (0.055 mole) of aqueous 35% formaldehyde. T...
10.6084/m9.figshare.5104873.v1
null
Formaldehyde.Primary amine.Sulfinic acid
Tosylate.Secondary amine
null
null
c1ncncn1.c1ccccc1
HO-
O.CO
null
0.5
C=O.COc1nc(N)nc(N(C)C)n1.Cc1ccc(S(=O)O)cc1>O.CO>COc1nc(NCS(=O)(=O)c2ccc(C)cc2)nc(N(C)C)n1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-9ea8c5f23c574b2e8a2a3b12fa410e55
C=O.Cc1cc(C)nc(N)n1.Cc1cccc(S(=O)(=O)O)c1>>Cc1ccc(S(=O)(=O)CNc2nc(C)cc(C)n2)cc1
NC1=NC(=CC(=N1)C)C.CS(=O)(=O)O.C1(=CC(=CC=C1)S(=O)(=O)O)C.[Na].C=O>>CC1=NC(=NC(=C1)C)NCS(=O)(=O)C1=CC=C(C=C1)C
O=[CH2:9].[NH2:10][c:11]1[n:12][c:13]([CH3:14])[cH:15][c:16]([CH3:17])[n:18]1.O[S:6](=[O:7])(=[O:8])[c:19]1[cH:5][cH:4][cH:3][c:2]([CH3:1])[cH:20]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([S:6](=[O:7])(=[O:8])[CH2:9][NH:10][c:11]2[n:12][c:13]([CH3:14])[cH:15][c:16]([CH3:17])[n:18]2)[cH:19][cH:20]1
C=O.Cc1cc(C)nc(N)n1.Cc1cccc(S(=O)(=O)O)c1
Cc1ccc(S(=O)(=O)CNc2nc(C)cc(C)n2)cc1
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
7bba7f008d6d215a625995cd0c52299c1a291736daf4b92e547b292fd3935501
b8d22e398bb2141ed6bf44c041465a74f13a3a3980569b6b5ed75cf915e69b0a
O=S(=O)(CNc1ncccn1)c1ccccc1
O-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c;H0;D3;+0:4]1:[c:5]:[c:6]:[c:7]:[c:8]:[cH;D2;+0:9]:1.O=[CH2;D1;+0:10].[NH2;D1;+0:11]-[c:12](:[#7;a:13]:[c:14]):[#7;a:15]:[c:16]>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[CH2;D2;+0:10]-[NH;D2;+0:11]-[c:12](:[#7;a:13]:[c:14]):[#7;a:15]:[c:16])-[c;H0;D3;+0:9]1:[c:8]:[c:7]:[...
null
[]
90
CELSIUS
30
MINUTE
12.7 g (0.1 mole) of 2-amino-4,6-dimethylpyrimidine are suspended in 200 ml of water and then 9.7 g (0.1 mole) of methanesulfonic acid are stirred in to form a solution. To the stirred solution are added, in succession, 18.22 g (0.1 mole) of toluene-3-sulfonic acid, sodium salt, and 9.4 g (0.11 mole) of aqueous 35% for...
10.6084/m9.figshare.5104873.v1
null
Formaldehyde.Primary amine.Sulfonic acid
Tosylate.Secondary amine
c1ccccc1
c1ccccc1
c1ccccc1.c1cncnc1
HO-
O
90
0.5
C=O.Cc1cc(C)nc(N)n1.Cc1cccc(S(=O)(=O)O)c1>O>Cc1ccc(S(=O)(=O)CNc2nc(C)cc(C)n2)cc1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-78661fbdfa654983baaed09f4ca62550
C1COCCN1.C=O.Cc1cc(C)nc(N)n1.S=C=S>>Cc1cc(C)nc(NCSC(=S)N2CCOCC2)n1
[OH-].[K+].N1CCOCC1.C=O.NC1=NC(=CC(=N1)C)C.CS(=O)(=O)O.C(=S)=S>>CC1=NC(=NC(=C1)C)NCSC(=S)N1CCOCC1
[NH:13]1[CH2:14][CH2:15][O:16][CH2:17][CH2:18]1.O=[CH2:9].[CH3:1][c:2]1[cH:3][c:4]([CH3:5])[n:6][c:7]([NH2:8])[n:19]1.[S:10]=[C:11]=[S:12]>>[CH3:1][c:2]1[cH:3][c:4]([CH3:5])[n:6][c:7]([NH:8][CH2:9][S:10][C:11](=[S:12])[N:13]2[CH2:14][CH2:15][O:16][CH2:17][CH2:18]2)[n:19]1
C1COCCN1.C=O.Cc1cc(C)nc(N)n1.S=C=S
Cc1cc(C)nc(NCSC(=S)N2CCOCC2)n1
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
622ede3764689099a2c31b37fbc8717beac4ccad2e490216abada1042cfab33f
80788209fd0aae246bafc18ed21d4b215eaa8c214878a69f8c868fb82a169d89
S=C(SCNc1ncccn1)N1CCOCC1
O=[CH2;D1;+0:1].[#8:2]1-[C:3]-[C:4]-[NH;D2;+0:5]-[C:6]-[C:7]-1.[NH2;D1;+0:8]-[c:9](:[#7;a:10]:[c:11]):[#7;a:12]:[c:13].[S;D1;H0:14]=[C;H0;D2;+0:15]=[S;H0;D1;+0:16]>>[S;D1;H0:14]=[C;H0;D3;+0:15](-[S;H0;D2;+0:16]-[CH2;D2;+0:1]-[NH;D2;+0:8]-[c:9](:[#7;a:10]:[c:11]):[#7;a:12]:[c:13])-[N;H0;D3;+0:5]1-[C:4]-[C:3]-[#8:2]-[C:7...
null
[]
null
null
null
null
6.6 g (0.1 mole) of 85% potassium hydroxide and 8.9 g (0.1 mole) of morpholine are dissolved in 200 ml of water and, with cooling, 7.7 g (0.1 mole) of carbon disulfide are added. The mixture is stirred until a yellowish homogeneous solution is obtained. With cooling and stirring, 9.4 g (0.11 mole) of aqueous 35% formal...
10.6084/m9.figshare.5104873.v1
null
Formaldehyde.Primary amine.Secondary amine
Thioamide.Secondary amine.Monosulfide
C1COCCN1
C1COCC[NH]1
c1cncnc1.C1COCC[NH]1
HO-
O
null
null
C1COCCN1.C=O.Cc1cc(C)nc(N)n1.S=C=S>O>Cc1cc(C)nc(NCSC(=S)N2CCOCC2)n1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-e6ac12f889244b25b87f4427cb95a90e
C=O.COc1cc(C)nc(N)n1.c1nc[nH]n1>>COc1cc(C)nc(NCn2cncn2)n1
NC1=NC(=CC(=N1)OC)C.N1N=CN=C1.C=O.C(C)(=O)O>>COC1=NC(=NC(=C1)C)NCN1N=CN=C1
O=[CH2:10].[CH3:1][O:2][c:3]1[cH:4][c:5]([CH3:6])[n:7][c:8]([NH2:9])[n:16]1.[nH:11]1[cH:12][n:13][cH:14][n:15]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]([CH3:6])[n:7][c:8]([NH:9][CH2:10][n:11]2[cH:12][n:13][cH:14][n:15]2)[n:16]1
C=O.COc1cc(C)nc(N)n1.c1nc[nH]n1
COc1cc(C)nc(NCn2cncn2)n1
null
null
CO
Heteroatom Alkylation and Arylation
OtherReaction
8c84100e28a403468c817276a093b527e625f7bba994cd1da5e6792c1b1cf4c1
cf32f1267c674fd84d46b8a676a46bd4e3a018dea282d34ea9ab93d79b66d0ee
c1cnc(NCn2cncn2)nc1
O=[CH2;D1;+0:1].[#7;a:2]1:[c:3]:[nH;D2;+0:4]:[#7;a:5]:[c:6]:1.[NH2;D1;+0:7]-[c:8](:[#7;a:9]:[c:10]):[#7;a:11]:[c:12]>>[c:10]:[#7;a:9]:[c:8](-[NH;D2;+0:7]-[CH2;D2;+0:1]-[n;H0;D3;+0:4]1:[#7;a:5]:[c:6]:[#7;a:2]:[c:3]:1):[#7;a:11]:[c:12]
null
[]
null
null
null
null
With stirring, a mixture of 13.9 g (0.1 mole) of 2-amino-4-methoxy-6-methylpyrimidine, 7 g (0.1 mole) of 1,2,4,-triazole, 9.4 g (0.11 mole) of aqueous 35% formaldehyde and 1 g of acetic acid in 100 ml of methanol is refluxed for 11/2 hours. First a clear solution forms, from which the reaction product precipitates in c...
10.6084/m9.figshare.5104873.v1
null
Formaldehyde.Primary amine
Secondary amine
c1nc[nH]n1
c1nc[nH]n1
c1cncnc1.c1nc[nH]n1
HO-
CO
null
null
C=O.COc1cc(C)nc(N)n1.c1nc[nH]n1>CO>COc1cc(C)nc(NCn2cncn2)n1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-96190d336abf42e882d1fda197689a7c
C=O.COc1nc(N)nc(N(C)C)n1.c1ccc2[nH]nnc2c1>>COc1nc(NCn2nnc3ccccc32)nc(N(C)C)n1
NC1=NC(=NC(=N1)N(C)C)OC.N1N=NC2=C1C=CC=C2.C=O.C(C)(=O)O>>N1(N=NC2=C1C=CC=C2)CNC2=NC(=NC(=N2)N(C)C)OC
O=[CH2:7].[CH3:1][O:2][c:3]1[n:4][c:5]([NH2:6])[n:17][c:18]([N:19]([CH3:20])[CH3:21])[n:22]1.[nH:8]1[n:9][n:10][c:11]2[cH:12][cH:13][cH:14][cH:15][c:16]12>>[CH3:1][O:2][c:3]1[n:4][c:5]([NH:6][CH2:7][n:8]2[n:9][n:10][c:11]3[cH:12][cH:13][cH:14][cH:15][c:16]23)[n:17][c:18]([N:19]([CH3:20])[CH3:21])[n:22]1
C=O.COc1nc(N)nc(N(C)C)n1.c1ccc2[nH]nnc2c1
COc1nc(NCn2nnc3ccccc32)nc(N(C)C)n1
null
null
C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
964b08c92ca6a1eb522d1beec780c5667fd2506de546d8bb86662dc90843a206
cf32f1267c674fd84d46b8a676a46bd4e3a018dea282d34ea9ab93d79b66d0ee
c1ccc2c(c1)nnn2CNc1ncncn1
O=[CH2;D1;+0:1].[NH2;D1;+0:2]-[c:3]1:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:[#7;a:8]:1.[c:9]:[c:10]1:[#7;a:11]:[#7;a:12]:[nH;D2;+0:13]:[c:14]:1:[c:15]>>[c:9]:[c:10]1:[#7;a:11]:[#7;a:12]:[n;H0;D3;+0:13](-[CH2;D2;+0:1]-[NH;D2;+0:2]-[c:3]2:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:[#7;a:8]:2):[c:14]:1:[c:15]
null
[]
null
null
null
null
With stirring, a mixture of 16.9 g (0.1 mole) of 2-amino-4-dimethylamino-6-methoxy-1,3,5-triazine, 12 g (0.1 mole) of benztriazole, 9.4 g (0.11 mole) of aqueous 35% formaldehyde and 1 g of acetic acid in 100 ml of ethanol is heated under reflux for 2 hours. The still hot solution is clarified by filtration and crystals...
10.6084/m9.figshare.5104873.v1
null
Formaldehyde.Primary amine
Secondary amine
c1ccc2[nH]nnc2c1
c1ccc2[nH]nnc2c1
c1ncncn1.c1ccc2[nH]nnc2c1
HO-
C(C)O
null
null
C=O.COc1nc(N)nc(N(C)C)n1.c1ccc2[nH]nnc2c1>C(C)O>COc1nc(NCn2nnc3ccccc32)nc(N(C)C)n1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-9db9650dad6b4080bfc625b5cf3e8620
Cc1cc(C)nc(NCn2cncn2)n1.O=C=NS(=O)(=O)c1ccccc1Cl>>Cc1cc(C)nc(N(Cn2cncn2)C(=O)NS(=O)(=O)c2ccccc2Cl)n1
N1(N=CN=C1)CNC1=NC(=CC(=N1)C)C.ClC1=C(C=CC=C1)S(=O)(=O)N=C=O>>ClC1=C(C=CC=C1)S(=O)(=O)NC(=O)N(C1=NC(=CC(=N1)C)C)CN1N=CN=C1
[CH3:1][c:2]1[cH:3][c:4]([CH3:5])[n:6][c:7]([NH:8][CH2:9][n:10]2[cH:11][n:12][cH:13][n:14]2)[n:28]1.[C:15](=[O:16])=[N:17][S:18](=[O:19])(=[O:20])[c:21]1[cH:22][cH:23][cH:24][cH:25][c:26]1[Cl:27]>>[CH3:1][c:2]1[cH:3][c:4]([CH3:5])[n:6][c:7]([N:8]([CH2:9][n:10]2[cH:11][n:12][cH:13][n:14]2)[C:15](=[O:16])[NH:17][S:18](=[...
Cc1cc(C)nc(NCn2cncn2)n1.O=C=NS(=O)(=O)c1ccccc1Cl
Cc1cc(C)nc(N(Cn2cncn2)C(=O)NS(=O)(=O)c2ccccc2Cl)n1
null
null
C(C)#N
Acylation
Urea synthesis via isocyanate and secondary amine
80efce6ceeace49536a85672860e2a5e31d8b9c94341eecb2be7c2c049271cea
c54c1ed6f5693fe7284d99bae8ce6ef1af2bc669c2b604d5d1041c83f556df82
O=C(NS(=O)(=O)c1ccccc1)N(Cn1cncn1)c1ncccn1
[#7;a:1]-[C:2]-[NH;D2;+0:3]-[c:4](:[#7;a:5]:[c:6]):[#7;a:7]:[c:8].[O;D1;H0:9]=[C;H0;D2;+0:10]=[N;H0;D2;+0:11]-[#16:12](=[O;D1;H0:13])(=[O;D1;H0:14])-[c:15]>>[#7;a:1]-[C:2]-[N;H0;D3;+0:3](-[C;H0;D3;+0:10](=[O;D1;H0:9])-[NH;D2;+0:11]-[#16:12](=[O;D1;H0:13])(=[O;D1;H0:14])-[c:15])-[c:4](:[#7;a:5]:[c:6]):[#7;a:7]:[c:8]
62.4
[{"value": 62.0, "product": "ClC1=C(C=CC=C1)S(=O)(=O)NC(=O)N(C1=NC(=CC(=N1)C)C)CN1N=CN=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 62.4, "product": "ClC1=C(C=CC=C1)S(=O)(=O)NC(=O)N(C1=NC(=CC(=N1)C)C)CN1N=CN=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
24
HOUR
4 g (0.019 mole) of 2-(1,2,4-triazol-1-ylmethylamino)-4,6-dimethylpyrimidine are suspended in 100 ml of absolute acetonitrile and then 4.3 g (0.019 mole) of 2-chlorophenylsulfonylisocyanate are stirred into the suspension. The batch is stirred for 24 hours at room temperature and the resultant solution is finally conce...
10.6084/m9.figshare.5104873.v1
null
Secondary amine
Sulfonamide.Urea
null
null
c1cncnc1.c1nc[nH]n1.c1ccccc1
null
C(C)#N
null
24
Cc1cc(C)nc(NCn2cncn2)n1.O=C=NS(=O)(=O)c1ccccc1Cl>C(C)#N>Cc1cc(C)nc(N(Cn2cncn2)C(=O)NS(=O)(=O)c2ccccc2Cl)n1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-ed5ce096de33477dad5a1554e18687b9
CC(C)(C)NS(=O)(=O)c1ccccc1C=C1CCOC1=O>>NS(=O)(=O)c1ccccc1C=C1CCOC1=O
CC(C)(C)NS(=O)(=O)C1=C(C=CC=C1)C=C1C(OCC1)=O>>O=C1OCCC1=CC1=C(C=CC=C1)S(=O)(=O)N
CC(C)(C)[NH:1][S:2](=[O:3])(=[O:4])[c:5]1[cH:6][cH:7][cH:8][cH:9][c:10]1[CH:11]=[C:12]1[CH2:13][CH2:14][O:15][C:16]1=[O:17]>>[NH2:1][S:2](=[O:3])(=[O:4])[c:5]1[cH:6][cH:7][cH:8][cH:9][c:10]1[CH:11]=[C:12]1[CH2:13][CH2:14][O:15][C:16]1=[O:17]
CC(C)(C)NS(=O)(=O)c1ccccc1C=C1CCOC1=O
NS(=O)(=O)c1ccccc1C=C1CCOC1=O
null
null
FC(C(=O)O)(F)F
Deprotection
Tert-butyl deprotection of amine
f7e1da1b4c254f1e6d5afbf8cb56733a4fabd145b80e971e3b7e31007de9e7d6
278d0fb11b582c058ac903379d7fbe11ab8c395937a204965031cf0c344845a9
O=C1OCCC1=Cc1ccccc1
C-C(-C)(-C)-[NH;D2;+0:1]-[#16:2](=[O;D1;H0:3])(=[O;D1;H0:4])-[c:5]>>[NH2;D1;+0:1]-[#16:2](=[O;D1;H0:3])(=[O;D1;H0:4])-[c:5]
88.8
[{"value": 88.0, "product": "O=C1OCCC1=CC1=C(C=CC=C1)S(=O)(=O)N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 88.8, "product": "O=C1OCCC1=CC1=C(C=CC=C1)S(=O)(=O)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 5.0 g (0.016 mol) of the product of Example 2 in 70 mL trifluoroacetic acid was stirred at room temperature overnight and was then evaporated to yield 3.6 g (88%) of the title compound: m.p. 178°-180°; IR (nujol) 3330, 3230, 3220, 1720, 1640, 1340, 1160 cm-1 ; NMR (DMSO-d6, 200 MHz) δ 3.12 (2H, m), 4.36 (...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide
Sulfonamide
null
null
c1ccccc1.C1CCOC1
Other
FC(C(=O)O)(F)F
null
null
CC(C)(C)NS(=O)(=O)c1ccccc1C=C1CCOC1=O>FC(C(=O)O)(F)F>NS(=O)(=O)c1ccccc1C=C1CCOC1=O
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-248ffe0971b44f2582d70db20b332f12
COc1cc(OC)nc(NC(=O)Oc2ccccc2)n1.NS(=O)(=O)c1ccccc1C=C1CCOC1=O>>COc1cc(OC)nc(NC(=O)NS(=O)(=O)c2ccccc2C=C2CCOC2=O)n1
Cl.O=C1OCCC1=CC1=C(C=CC=C1)S(=O)(=O)N.COC1=NC(=NC(=C1)OC)NC(OC1=CC=CC=C1)=O.N12CCCCCC2=NCCC1>>COC1=NC(=NC(=C1)OC)NC(=O)NS(=O)(=O)C1=C(C=CC=C1)C=C1C(OCC1)=O
c1ccc(O[C:11]([NH:10][c:9]2[n:8][c:5]([O:6][CH3:7])[cH:4][c:3]([O:2][CH3:1])[n:30]2)=[O:12])cc1.[NH2:13][S:14](=[O:15])(=[O:16])[c:17]1[cH:18][cH:19][cH:20][cH:21][c:22]1[CH:23]=[C:24]1[CH2:25][CH2:26][O:27][C:28]1=[O:29]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([O:6][CH3:7])[n:8][c:9]([NH:10][C:11](=[O:12])[NH:13][S:14](=[O:15]...
COc1cc(OC)nc(NC(=O)Oc2ccccc2)n1.NS(=O)(=O)c1ccccc1C=C1CCOC1=O
COc1cc(OC)nc(NC(=O)NS(=O)(=O)c2ccccc2C=C2CCOC2=O)n1
null
null
C(C)#N.O
Acylation
OtherReaction
667fe6067474f88ffbad5ef8e75ea479abb1dcdb90207bfe1bf5fbbda20a2b82
7357574545fa4eeb65dbf65b1651a3185814d8225c8c3386649f2331a5a0c761
O=C(Nc1ncccn1)NS(=O)(=O)c1ccccc1C=C1CCOC1=O
[#7;a:1]:[c:2](-[#7:3]-[C;H0;D3;+0:4](=[O;D1;H0:5])-O-c1:c:c:c:c:c:1):[#7;a:6].[NH2;D1;+0:7]-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11]>>[#7;a:1]:[c:2](-[#7:3]-[C;H0;D3;+0:4](=[O;D1;H0:5])-[NH;D2;+0:7]-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11]):[#7;a:6]
64
[{"value": 64.0, "product": "COC1=NC(=NC(=C1)OC)NC(=O)NS(=O)(=O)C1=C(C=CC=C1)C=C1C(OCC1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 57.5, "product": "COC1=NC(=NC(=C1)OC)NC(=O)NS(=O)(=O)C1=C(C=CC=C1)C=C1C(OCC1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
To a stirred suspension of 0.09 g (0.0004 mol) of the product of Example 3 and 0.15 g (0.0005 mol) of (4,6-dimethoxy-2-pyrimidinyl)carbamic acid, phenyl ester in 1 mL dry acetonitrile under nitrogen was added dropwise 0.08 mL (0.08 g, 0.0005 mol) of 1,8-diazabicyclo[5.4.0]undec-7-ene. The mixture was stirred at room te...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Carbamic ester.Ether
Sulfonamide.Urea
c1ccccc1
null
c1cncnc1.c1ccccc1.C1CCOC1
HO-
C(C)#N.O
null
0.5
COc1cc(OC)nc(NC(=O)Oc2ccccc2)n1.NS(=O)(=O)c1ccccc1C=C1CCOC1=O>C(C)#N.O>COc1cc(OC)nc(NC(=O)NS(=O)(=O)c2ccccc2C=C2CCOC2=O)n1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-ce37ff459f5848f19fc1dbc7eb1ac0e2
COc1cc(OC)nc(NC(=O)Oc2ccccc2)n1.NS(=O)(=O)c1cccc(Cl)c1C=C1CCOC1=O>>COc1cc(OC)nc(NC(=O)NS(=O)(=O)c2cccc(Cl)c2C=C2CCOC2=O)n1
Cl.ClC=1C(=C(C=CC1)S(=O)(=O)N)C=C1C(OCC1)=O.COC1=NC(=NC(=C1)OC)NC(OC1=CC=CC=C1)=O.N12CCCCCC2=NCCC1>>ClC=1C(=C(C=CC1)S(=O)(=O)NC(=O)NC1=NC(=CC(=N1)OC)OC)C=C1C(OCC1)=O
c1ccc(O[C:11]([NH:10][c:9]2[n:8][c:5]([O:6][CH3:7])[cH:4][c:3]([O:2][CH3:1])[n:31]2)=[O:12])cc1.[NH2:13][S:14](=[O:15])(=[O:16])[c:17]1[cH:18][cH:19][cH:20][c:21]([Cl:22])[c:23]1[CH:24]=[C:25]1[CH2:26][CH2:27][O:28][C:29]1=[O:30]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([O:6][CH3:7])[n:8][c:9]([NH:10][C:11](=[O:12])[NH:13][S:14]...
COc1cc(OC)nc(NC(=O)Oc2ccccc2)n1.NS(=O)(=O)c1cccc(Cl)c1C=C1CCOC1=O
COc1cc(OC)nc(NC(=O)NS(=O)(=O)c2cccc(Cl)c2C=C2CCOC2=O)n1
null
null
C(C)#N.O
Acylation
OtherReaction
667fe6067474f88ffbad5ef8e75ea479abb1dcdb90207bfe1bf5fbbda20a2b82
7357574545fa4eeb65dbf65b1651a3185814d8225c8c3386649f2331a5a0c761
O=C(Nc1ncccn1)NS(=O)(=O)c1ccccc1C=C1CCOC1=O
[#7;a:1]:[c:2](-[#7:3]-[C;H0;D3;+0:4](=[O;D1;H0:5])-O-c1:c:c:c:c:c:1):[#7;a:6].[NH2;D1;+0:7]-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11]>>[#7;a:1]:[c:2](-[#7:3]-[C;H0;D3;+0:4](=[O;D1;H0:5])-[NH;D2;+0:7]-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11]):[#7;a:6]
85.3
[{"value": 83.0, "product": "ClC=1C(=C(C=CC1)S(=O)(=O)NC(=O)NC1=NC(=CC(=N1)OC)OC)C=C1C(OCC1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 85.3, "product": "ClC=1C(=C(C=CC1)S(=O)(=O)NC(=O)NC1=NC(=CC(=N1)OC)OC)C=C1C(OCC1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a stirred suspension of 0.15 g (0.0005 mol) of the product of Example 7 and 0.21 g (0.0008 mol) of (4,6-dimethoxy-2-pyrimidinyl)carbamic acid, phenyl ester in 1 mL dry acetonitrile under nitrogen was added dropwise 0.12 mL (0.12 g, 0.0008 mol) of 1,8-diazabicyclo[5.4.0]undec-7-ene. The mixture was stirred at room te...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Carbamic ester.Ether
Sulfonamide.Urea
c1ccccc1
null
c1cncnc1.c1ccccc1.C1CCOC1
HO-
C(C)#N.O
null
1
COc1cc(OC)nc(NC(=O)Oc2ccccc2)n1.NS(=O)(=O)c1cccc(Cl)c1C=C1CCOC1=O>C(C)#N.O>COc1cc(OC)nc(NC(=O)NS(=O)(=O)c2cccc(Cl)c2C=C2CCOC2=O)n1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-132d57a3cbc44f74a5722eea269ca6a1
C1CO1.CN(C)C.CN(C)C.O>>C=O.C[N+](C)(C)CCO
CN(C)C.C1CO1.CN(C)C.O>>OCC[N+](C)(C)C.C=O
[CH2:1]1[O:2][CH2:8]1.[CH3:3][N:4]([CH3:6])[CH3:7].CN(C)[CH3:5].[OH2:9]>>[CH2:1]=[O:2].[CH3:3][N+:4]([CH3:5])([CH3:6])[CH2:7][CH2:8][OH:9]
C1CO1.CN(C)C.CN(C)C.O
C=O.C[N+](C)(C)CCO
null
null
CO
Acylation
OtherReaction
c4cae58d4998d89ea221170ced61c2f4e01f2f1a5c40e1945038df4cf31725ca
d5f253a16a8cbc6a682b244c7c69606dd4698869e69432db144dfe507f28473e
null
C-N(-C)-[CH3;D1;+0:1].[C;D1;H3:2]-[N;H0;D3;+0:3](-[C;D1;H3:4])-[CH3;D1;+0:5].[CH2;D2;+0:6]1-[CH2;D2;+0:7]-[O;H0;D2;+0:8]-1.[OH2;D0;+0:9]>>[C;D1;H3:2]-[N+;H0;D4:3](-[C;D1;H3:4])(-[CH3;D1;+0:1])-[CH2;D2;+0:5]-[CH2;D2;+0:7]-[OH;D1;+0:9].[CH2;D1;+0:6]=[O;H0;D1;+0:8]
null
[]
null
null
null
null
45% by weight choline base in methanol was prepared by the reaction of ethylene oxide with a methanolic solution of 1:1 trimethylamine/water. The trimethylamine content of the stock solution as prepared was 19 ppm. Sufficient paraformaldehyde to give solutions containing 0.05%, 0.1%, 0.5%, and 1% by weight of paraforma...
10.6084/m9.figshare.5104873.v1
null
Ether.Tertiary amine.Tertiary amine
Formaldehyde.Primary alcohol
C1CO1
null
null
Other
CO
null
null
C1CO1.CN(C)C.CN(C)C.O>CO>C=O.C[N+](C)(C)CCO
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-847683fa01a94eecbf93753ed93e77bd
Cc1ccc(O)cc1.OO>>Cc1ccc(O)c(O)c1
OO.OO.C1=CC(=CC=C1O)C>>CC=1C=C(C(O)=CC1)O
[CH3:1][c:2]1[cH:3][cH:4][c:5]([OH:6])[cH:7][cH:9]1.O[OH:8]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([OH:6])[c:7]([OH:8])[cH:9]1
Cc1ccc(O)cc1.OO
Cc1ccc(O)c(O)c1
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
ae2c40671d5fdb818f0b6d803c1d8cceca080b6105aceeca1808a097ec52d441
a2fdf414569b219d462bc05c91ebf31e5426b96645f5c78cb091f50cc92fc345
c1ccccc1
O-[OH;D1;+0:1].[O;D1;H1:2]-[c:3](:[c:4]):[cH;D2;+0:5]:[c:6]:[c:7]>>[O;D1;H1:2]-[c:3](:[c:4]):[c;H0;D3;+0:5](-[OH;D1;+0:1]):[c:6]:[c:7]
65.1
[{"value": 65.1, "product": "CC=1C=C(C(O)=CC1)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
A water-free solution of 3.40 grams of H2O2 (0.1 mole) in 108.1 grams (1.0 mole) of p-cresol was heated to 95° C. and treated with 0.018 gram (0.00015 mole) of SeO2. The temperature increased in connection therewith to 161° C. After 15 minutes there was determined a hydrogen peroxide reaction of 99.4%. At that time the...
10.6084/m9.figshare.5104873.v1
null
Peroxide
Aromatic alcohol
c1ccccc1
c1ccccc1
c1ccccc1
HO-
O
null
0.25
Cc1ccc(O)cc1.OO>O>Cc1ccc(O)c(O)c1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-bf696a9a0941417da664285712a10733
FC1(F)C(Cl)=C(Cl)C(F)(F)C1(F)F.OC1CCCC1>>FC1(F)C(Cl)=C(OC2CCCC2)C(F)(F)C1(F)F
C1(CCCC1)O.[Na].O1CCCC1.ClC1=C(C(C(C1(F)F)(F)F)(F)F)Cl>>C1(CCCC1)OC1=C(C(C(C1(F)F)(F)F)(F)F)Cl
Cl[C:6]1=[C:4]([Cl:5])[C:2]([F:1])([F:3])[C:16]([F:17])([F:18])[C:13]1([F:14])[F:15].[OH:7][CH:8]1[CH2:9][CH2:10][CH2:11][CH2:12]1>>[F:1][C:2]1([F:3])[C:4]([Cl:5])=[C:6]([O:7][CH:8]2[CH2:9][CH2:10][CH2:11][CH2:12]2)[C:13]([F:14])([F:15])[C:16]1([F:17])[F:18]
FC1(F)C(Cl)=C(Cl)C(F)(F)C1(F)F.OC1CCCC1
FC1(F)C(Cl)=C(OC2CCCC2)C(F)(F)C1(F)F
null
null
CCOCC
Acylation
Williamson Ether Synthesis
e1886bb86311b4c11f16e746fcfb243de4783d54bc2b43a5210a5ef250fe1061
8b2d7ad98b9e5b3aa4ef11010bc628a0a98442b0fea590e26be12d72c542b653
C1=C(OC2CCCC2)CCC1
Cl-[C;H0;D3;+0:1]1=[C:2](-[Cl;D1;H0:3])-[C:4]-[C:5]-[C:6]-1(-[F;D1;H0:7])-[F;D1;H0:8].[C:9]-[C:10](-[OH;D1;+0:11])-[C:12]>>[C:9]-[C:10](-[O;H0;D2;+0:11]-[C;H0;D3;+0:1]1=[C:2](-[Cl;D1;H0:3])-[C:4]-[C:5]-[C:6]-1(-[F;D1;H0:7])-[F;D1;H0:8])-[C:12]
79
[{"value": 79.0, "product": "C1(CCCC1)OC1=C(C(C(C1(F)F)(F)F)(F)F)Cl", "details": "PERCENTYIELD", "is_desired": false}]
null
null
20
MINUTE
Cyclopentanol (23 g, 0.27 mol) and sodium metal (5.6 g, 0.24 mol) were refluxed with 25 ml dry tetrahydrofuran (THF) overnight. The reaction mixture was diluted with 200 ml of dry ether and then added to 1,2-dichlorohexafluorocyclopentene (49 g, 0.2 mol) in 100 ml of dry ether at room temperature with stirring over 20 ...
10.6084/m9.figshare.5104873.v1
null
Alkenyl halide.Secondary alcohol
Ether
C1=CCCC1
C1=CCCC1
C1=CCCC1.C1CCCC1
HCl
CCOCC
null
0.333333
FC1(F)C(Cl)=C(Cl)C(F)(F)C1(F)F.OC1CCCC1>CCOCC>FC1(F)C(Cl)=C(OC2CCCC2)C(F)(F)C1(F)F
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-8a125ea60f50441aa95a30af6dfecf36
CCCCCCCCCN.O=C1CCC(=O)O1>>CCCCCCCCCNC(=O)CCC(=O)O
C1(CCC(=O)O1)=O.C(CCCCCCCC)N>>C(CCCCCCCC)NC(CCC(=O)O)=O
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][NH2:10].[C:11]1(=[O:12])[CH2:13][CH2:14][C:15](=[O:16])[O:17]1>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][NH:10][C:11](=[O:12])[CH2:13][CH2:14][C:15](=[O:16])[OH:17]
CCCCCCCCCN.O=C1CCC(=O)O1
CCCCCCCCCNC(=O)CCC(=O)O
null
null
CC(=O)C
Protection
OtherReaction
058bd4c79f70dc248cff01dbd6bcb24847e7daaca3b07e9cb2eccef1b565fa6e
d83a5fe7c1575bfa4f6a9dc1cf7406e299c5c7ecfc75f13bc6d348857a70653f
null
[C:1]-[C:2]-[NH2;D1;+0:3].[O;D1;H0:4]=[C;H0;D3;+0:5]1-[C:6]-[C:7]-[C:8](=[O;D1;H0:9])-[O;H0;D2;+0:10]-1>>[C:1]-[C:2]-[NH;D2;+0:3]-[C;H0;D3;+0:5](=[O;D1;H0:4])-[C:6]-[C:7]-[C:8](=[O;D1;H0:9])-[OH;D1;+0:10]
79.7
[{"value": 79.7, "product": "C(CCCCCCCC)NC(CCC(=O)O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a stirred solution of succinic anhydride (25.0 g, 0.25 mol) in 150 mL acetone was added dropwise 35.8 g (0.25 mol) of nonylamine. The addition of the amine required 15 minutes, with the acetone solution reaching reflux before the addition was complete. Five minutes after the end of addition, a precipitate formed and...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Primary amine
Carboxylic acid.Secondary amide
C1CCOC1
null
null
null
CC(=O)C
null
1
CCCCCCCCCN.O=C1CCC(=O)O1>CC(=O)C>CCCCCCCCCNC(=O)CCC(=O)O
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-dfb6c7d8e04e492d834e68ed06daa65a
CCCCCCCCCNC(=O)CCC(=O)O.OO>>CCCCCCCCCNC(=O)CCC(=O)OO
C(CCCCCCCC)NC(CCC(=O)O)=O.OO>>C(CCCCCCCC)NC(CCC(=O)OO)=O
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][NH:10][C:11](=[O:12])[CH2:13][CH2:14][C:15](=[O:16])[OH:17].O[OH:18]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][NH:10][C:11](=[O:12])[CH2:13][CH2:14][C:15](=[O:16])[O:17][OH:18]
CCCCCCCCCNC(=O)CCC(=O)O.OO
CCCCCCCCCNC(=O)CCC(=O)OO
null
null
CS(=O)(=O)O
Miscellaneous
OtherReaction
b226d77ae30ca76c37fc9cde5a987164e66aa37df4d2cd5f82b4f127c5a14a47
db20d33edf4ed6ad1c56374c48bc4c8c17a482c7135e5fe809b17d99f36da805
null
O-[OH;D1;+0:1].[C:2]-[C:3](=[O;D1;H0:4])-[OH;D1;+0:5]>>[C:2]-[C:3](=[O;D1;H0:4])-[O;H0;D2;+0:5]-[OH;D1;+0:1]
89.3
[{"value": 89.3, "product": "C(CCCCCCCC)NC(CCC(=O)OO)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-15
CELSIUS
null
null
A 500 mL beaker was charged with 50.0 g (0.205 mol) of 4-nonylamino-4-oxobutyric acid and 100 mL of 98% methanesulfonic acid. The resulting solution was cooled in an ice bath and, with stirring, 38.8 g of 90% hydrogen peroxide (34.9 g, 1.03 mol of hydrogen peroxide) was added dropwise at a rate such that the temperatur...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Peroxide
Peroxide
null
null
null
HO-
CS(=O)(=O)O
-15
null
CCCCCCCCCNC(=O)CCC(=O)O.OO>CS(=O)(=O)O>CCCCCCCCCNC(=O)CCC(=O)OO
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-db3f623b9a90456fae3c2ef1e6893c91
CCCCCCCCCN.COC(=O)CCCCC(=O)Cl>>CCCCCCCCCNC(=O)CCCCC(=O)O
[OH-].[Na+].C(=O)(OC)CCCCC(=O)Cl.[OH-].[Na+].O.C(CCCCCCCC)N>>C(CCCCCCCC)NC(CCCCC(=O)O)=O
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][NH2:10].C[O:19][C:17]([CH2:16][CH2:15][CH2:14][CH2:13][C:11](Cl)=[O:12])=[O:18]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][NH:10][C:11](=[O:12])[CH2:13][CH2:14][CH2:15][CH2:16][C:17](=[O:18])[OH:19]
CCCCCCCCCN.COC(=O)CCCCC(=O)Cl
CCCCCCCCCNC(=O)CCCCC(=O)O
null
null
CCOCC
Acylation
OtherReaction
ef24946e812c58ec5646342efa5dafd5ed10bf586e98ff0052340ef0daf33e7e
5dbbcac586755560aba4a2c29e7a14cbdd68815807327d0e3fd0dd155b11b926
null
C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4].Cl-[C;H0;D3;+0:5](=[O;D1;H0:6])-[C:7]-[C:8].[C:9]-[C:10]-[NH2;D1;+0:11]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1].[C:8]-[C:7]-[C;H0;D3;+0:5](=[O;D1;H0:6])-[NH;D2;+0:11]-[C:10]-[C:9]
null
[]
null
null
null
null
A two liter beaker fitted with a mechanical stirrer, ice bath, and pH electrode, was charged with 700 mL of water and 89.4 g (0.624 mol) of nonylamine in 200 mL of ether. To this stirred mixture was added dropwise over a 30 minute period a solution of the above 5-carbomethoxyvaleryl chloride in 100 mL of ether. Concurr...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Ester.Primary amine
Carboxylic acid.Secondary amide
null
null
null
HCl
CCOCC
null
null
CCCCCCCCCN.COC(=O)CCCCC(=O)Cl>CCOCC>CCCCCCCCCNC(=O)CCCCC(=O)O
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-48cc3136eead4903b29f1eb676c3acbe
CCCCCCCCCCCCCCCCCC(=O)O.O=S(Cl)Cl>>CCCCCCCCCCCCCCCCCC(=O)Cl
C(CCCCCCCCCCCCCCCCC)(=O)O.S(=O)(Cl)Cl>>C(CCCCCCCCCCCCCCCCC)(=O)Cl
O[C:18]([CH2:17][CH2:16][CH2:15][CH2:14][CH2:13][CH2:12][CH2:11][CH2:10][CH2:9][CH2:8][CH2:7][CH2:6][CH2:5][CH2:4][CH2:3][CH2:2][CH3:1])=[O:19].O=S(Cl)[Cl:20]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][CH2:13][CH2:14][CH2:15][CH2:16][CH2:17][C:18](=[O:19])[Cl:20]
CCCCCCCCCCCCCCCCCC(=O)O.O=S(Cl)Cl
CCCCCCCCCCCCCCCCCC(=O)Cl
null
null
null
Functional Group Interconversion
Alcohol to chloride_SOCl2
c301c14a9dcd0670d52e8b77396cbe7fd8edeedd757bc43f4162ade1fc52fc93
787f545db5dc0b29dde55b5fbed7db8625b8055f49327f97ed4d83cc47c3af1d
null
Cl-S(=O)-[Cl;H0;D1;+0:1].O-[C;H0;D3;+0:2](=[O;D1;H0:3])-[C:4]-[C:5]>>[C:5]-[C:4]-[C;H0;D3;+0:2](-[Cl;H0;D1;+0:1])=[O;D1;H0:3]
null
[]
null
null
null
null
Stearic acid (25 g) was reacted with thionylchloride (30 g) to form stearoylchloride, which was further reacted with indigo (5.2 g) in pyridine to obtain N,N'-distearoylindigo in per se conventional manners. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Acyl halide
null
null
null
HCl
null
null
null
CCCCCCCCCCCCCCCCCC(=O)O.O=S(Cl)Cl>>CCCCCCCCCCCCCCCCCC(=O)Cl
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-50543bc6295b422e96997e76c434c439
C=C(C)C(=O)Cl.OCC(F)(F)C(F)C(F)(F)F>>C=C(C)C(=O)OCC(F)(F)C(F)C(F)(F)F
COC1=CC=C(OC)C=C1.C(C(=C)C)(=O)Cl.FC(CO)(C(C(F)(F)F)F)F>>C(C(=C)C)(=O)OCC(C(C(F)(F)F)F)(F)F
Cl[C:4]([C:2](=[CH2:1])[CH3:3])=[O:5].[OH:6][CH2:7][C:8]([F:9])([F:10])[CH:11]([F:12])[C:13]([F:14])([F:15])[F:16]>>[CH2:1]=[C:2]([CH3:3])[C:4](=[O:5])[O:6][CH2:7][C:8]([F:9])([F:10])[CH:11]([F:12])[C:13]([F:14])([F:15])[F:16]
C=C(C)C(=O)Cl.OCC(F)(F)C(F)C(F)(F)F
C=C(C)C(=O)OCC(F)(F)C(F)C(F)(F)F
null
null
null
Acylation
Schotten-Baumann to ester
6cefe709828c5bd4655f254e75d5dff9e8876e192e7dd47256c1bc0067bc5291
d8a7643b81ed07a6f633aa99465180dfa0565e61ae25aef36338ebb9837c9cef
null
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](=[C;D1;H2:4])-[C;D1;H3:5].[C:6]-[C:7]-[OH;D1;+0:8]>>[C:6]-[C:7]-[O;H0;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](=[C;D1;H2:4])-[C;D1;H3:5]
null
[]
null
null
null
null
To 12 parts of methacrylic acid chloride were added 60 parts of 2,2,3,4,4,4-hexafluorobutyl alcohol as a reactant and a solvent and 0.1 part of hydroquinone dimethyl ether as a polymerization inhibitor. The mixture was heated at a temperature of 90° to 100° C. for 3 hours. The reaction mixture was distilled to give 15 ...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary alcohol
Ester
null
null
null
HCl
null
null
null
C=C(C)C(=O)Cl.OCC(F)(F)C(F)C(F)(F)F>>C=C(C)C(=O)OCC(F)(F)C(F)C(F)(F)F
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-a5d60f6518044b008e9086f16febeedf
CCc1c(Cl)cc([N+](=O)[O-])c(O)c1Cl>>CCc1c(Cl)cc(N)c(O)c1Cl.Cl
[N+](=O)([O-])C1=C(C(=C(C(=C1)Cl)CC)Cl)O>>Cl.NC1=C(C(=C(C(=C1)Cl)CC)Cl)O
O=[N+:8]([O-])[c:7]1[cH:6][c:4]([Cl:5])[c:3]([CH2:2][CH3:1])[c:11]([Cl:12])[c:9]1[OH:10]>>[CH3:1][CH2:2][c:3]1[c:4]([Cl:5])[cH:6][c:7]([NH2:8])[c:9]([OH:10])[c:11]1[Cl:12].[ClH:13]
CCc1c(Cl)cc([N+](=O)[O-])c(O)c1Cl
CCc1c(Cl)cc(N)c(O)c1Cl.Cl
null
[Ni]
C(C)(C)O
Functional Group Interconversion
Reduction of nitro groups to amines
5c1ea979989295c14f1f65f49e58974d5c524451abca65fc2e6cec44e3d0784f
10b8579fd1662beac4350d758bc16e1f45ee6ea295ff9572db62110c9e2a77db
c1ccccc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
525 ml of isopropyl alcohol, 125 g of the same 2-nitro-4,6-dichloro-5-ethylphenol as described above in (1) and 7.5 g of Raney nickel were placed in 1 liter of autoclave, and then the mixture was stirred until absorbing the theoretical amount of hydrogen gas under 10 kg/cm2 of initial pressure of hydrogen at 50° C. or ...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1
Other
[Ni].C(C)(C)O
null
null
CCc1c(Cl)cc([N+](=O)[O-])c(O)c1Cl>[Ni].C(C)(C)O>CCc1c(Cl)cc(N)c(O)c1Cl.Cl
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-036d8b08607c4f47ab181493a52479ca
COC(=O)Cc1occ(O)c2c3ccccc3nc1-2>>O=C(O)CC1=C2N=c3ccccc3=C2C(=O)CO1
COC(CC=1OC=C(C=2C1N=C1C=CC=CC21)O)=O>>O=C1COC(=C2N=C3C=CC=CC3=C21)CC(=O)O
C[O:3][C:2](=[O:1])[CH2:4][c:5]1[c:6]2[n:7][c:8]3[cH:9][cH:10][cH:11][cH:12][c:13]3[c:14]-2[c:15]([OH:16])[cH:17][o:18]1>>[O:1]=[C:2]([OH:3])[CH2:4][C:5]1=[C:6]2[N:7]=[c:8]3[cH:9][cH:10][cH:11][cH:12][c:13]3=[C:14]2[C:15](=[O:16])[CH2:17][O:18]1
COC(=O)Cc1occ(O)c2c3ccccc3nc1-2
O=C(O)CC1=C2N=c3ccccc3=C2C(=O)CO1
null
[O-2].[O-2].[Mn+4]
null
Reduction
OtherReaction
46c3591f22021913f3445ab6ce7ff044c9e99ac0449e68592c19e655b73f5c8b
2ae22b122b56b931fdbae62284a684d6d7c36387d89e3096cc7518e51dc2b69a
O=C1COC=C2N=c3ccccc3=C12
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[C:4]-[c;H0;D3;+0:5]1:[o;H0;D2;+0:6]:[cH;D2;+0:7]:[c;H0;D3;+0:8](-[OH;D1;+0:9]):[c;H0;D3;+0:10]2:[c;H0;D3;+0:11]3:[c:12]:[c:13]:[c:14]:[c:15]:[c;H0;D3;+0:16]:3:[n;H0;D2;+0:17]:[c;H0;D3;+0:18]:1-2>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[C:4]-[C;H0;D3;+0:5]1=[C;H0;D3;+0:18]2-[N;H0;D2;+0:17...
null
[]
null
null
null
null
Oxidation of 4-hydroxypyrano[3,4-b]indole acetic acid methyl ester 15 with manganese dioxide, followed by hydrolysis, afforded 4-oxopyrano[3,4-b]-indole acetic acid 18. When 15 was treated with urea in acidified aqueous tetrahydrofuran, a quantitative conversion to 4-ureidopyrano[3,4-b]indole acetic acid methyl ester 1...
10.6084/m9.figshare.5104873.v1
null
Ester.Aromatic alcohol
Carboxylic acid.Ketone.Ether
c1ccc2c(c1)nc1coccc12
C1=C2N=c3ccccc3=C2CCO1
C1=C2N=c3ccccc3=C2CCO1
Other
[O-2].[O-2].[Mn+4]
null
null
COC(=O)Cc1occ(O)c2c3ccccc3nc1-2>[O-2].[O-2].[Mn+4]>O=C(O)CC1=C2N=c3ccccc3=C2C(=O)CO1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-589aecb4d1ef418abc0ff082e9f786cc
CCOC(=O)C(=O)c1c[nH]c2c(CC)cccc12.NO>>CCOC(=O)C(=NO)c1c[nH]c2c(CC)cccc12
C(C)(=O)[O-].[Na+].Cl.NO.C(C)OC(C(C1=CNC2=C(C=CC=C12)CC)=O)=O>>C(C)OC(C(C1=CNC2=C(C=CC=C12)CC)=NO)=O
O=[C:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[c:9]1[cH:10][nH:11][c:12]2[c:13]([CH2:14][CH3:15])[cH:16][cH:17][cH:18][c:19]12.[NH2:7][OH:8]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[C:6](=[N:7][OH:8])[c:9]1[cH:10][nH:11][c:12]2[c:13]([CH2:14][CH3:15])[cH:16][cH:17][cH:18][c:19]12
CCOC(=O)C(=O)c1c[nH]c2c(CC)cccc12.NO
CCOC(=O)C(=NO)c1c[nH]c2c(CC)cccc12
null
null
O.C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
3b5816f78673484492f1e9027ec8b06843f9965cc3956d1b299528352460e3cb
d9a243f6ba886d56e0d31608707ecf09182055b9e74cac0b23531362bbd3484b
c1ccc2[nH]ccc2c1
O=[C;H0;D3;+0:1](-[C:2](=[O;D1;H0:3])-[#8:4]-[C:5])-[c:6]1:[c:7]:[#7;a:8]:[c:9]:[c:10]:1.[NH2;D1;+0:11]-[O;D1;H1:12]>>[C:5]-[#8:4]-[C:2](=[O;D1;H0:3])-[C;H0;D3;+0:1](=[N;H0;D2;+0:11]-[O;D1;H1:12])-[c:6]1:[c:7]:[#7;a:8]:[c:9]:[c:10]:1
75.7
[{"value": 75.0, "product": "C(C)OC(C(C1=CNC2=C(C=CC=C12)CC)=NO)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 75.7, "product": "C(C)OC(C(C1=CNC2=C(C=CC=C12)CC)=NO)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Solutions of sodium acetate (43.7 g, 0.53 mol) in water (100 mL) and hydroxylamine hydrochloride (37 g, 0.53 mol) in water (100 mL) were added to 7-ethyl-α-oxo-1H-indole-3-acetic acid ethyl ester 4 (17.4 g, 0.07 mol), in ethanol (250 mL) and the mixture was heated at reflux for 12 hours. The ethanol was removed by dist...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ester.Primary amine
Ester.Oxime
null
null
c1ccc2[nH]ccc2c1
HO-
O.C(C)O
null
null
CCOC(=O)C(=O)c1c[nH]c2c(CC)cccc12.NO>O.C(C)O>CCOC(=O)C(=NO)c1c[nH]c2c(CC)cccc12
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-bdf81a0e5dcd428ba7545489b8cf51ff
CCOC(=O)C(=NO)c1c[nH]c2c(CC)cccc12>>CCOC(=O)C(N)c1c[nH]c2c(CC)cccc12
C(C)OC(C(C1=CNC2=C(C=CC=C12)CC)=NO)=O.Cl>>C(C)OC(C(C1=CNC2=C(C=CC=C12)CC)N)=O
O[N:7]=[C:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[c:8]1[cH:9][nH:10][c:11]2[c:12]([CH2:13][CH3:14])[cH:15][cH:16][cH:17][c:18]12>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]([NH2:7])[c:8]1[cH:9][nH:10][c:11]2[c:12]([CH2:13][CH3:14])[cH:15][cH:16][cH:17][c:18]12
CCOC(=O)C(=NO)c1c[nH]c2c(CC)cccc12
CCOC(=O)C(N)c1c[nH]c2c(CC)cccc12
null
[Pd]
C(C)O
Reduction
OtherReaction
5ebe1a7876a79df84d3f4f7109df26bec79a6cac71893193e6457f66a461ae8a
ee0cd665e3f8693724283a166fc970d164796173c71ad91aea78c9e71235c1fa
c1ccc2[nH]ccc2c1
O-[N;H0;D2;+0:1]=[C;H0;D3;+0:2](-[C:3](=[O;D1;H0:4])-[#8:5]-[C:6])-[c:7]1:[c:8]:[c:9]:[#7;a:10]:[c:11]:1>>[C:6]-[#8:5]-[C:3](=[O;D1;H0:4])-[CH;D3;+0:2](-[NH2;D1;+0:1])-[c:7]1:[c:8]:[c:9]:[#7;a:10]:[c:11]:1
null
[]
null
null
4
HOUR
To 7-ethyl-α-(hydroxyimino)-1H-indole-3-acetic acid ethyl ester 5 (7.3 g, 0.028 mol) in ethanol (200 mL) was added concentrated HCl (3 mL) a nd 10% Pd/C (1.0 g). The mixture was hydrogenated at 40 p.s.i. for 4 hours at 22° C. The catalyst and the solvent were removed and the residue was dissolved in water. After washin...
10.6084/m9.figshare.5104873.v1
null
Ester.Oxime
Ester.Primary amine
null
null
c1ccc2[nH]ccc2c1
Other
[Pd].C(C)O
null
4
CCOC(=O)C(=NO)c1c[nH]c2c(CC)cccc12>[Pd].C(C)O>CCOC(=O)C(N)c1c[nH]c2c(CC)cccc12
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-5631154fce2f4da7b70e4f6954297de1
CCOC(=O)C(N)c1c[nH]c2c(CC)cccc12>>CCc1cccc2c(C(N)CO)c[nH]c12
C(C)OC(C(C1=CNC2=C(C=CC=C12)CC)N)=O.[H-].[H-].[H-].[H-].[Li+].[Al+3]>>NC(CO)C1=CNC2=C(C=CC=C12)CC
CCO[C:11]([CH:9]([c:8]1[c:7]2[cH:6][cH:5][cH:4][c:3]([CH2:2][CH3:1])[c:15]2[nH:14][cH:13]1)[NH2:10])=[O:12]>>[CH3:1][CH2:2][c:3]1[cH:4][cH:5][cH:6][c:7]2[c:8]([CH:9]([NH2:10])[CH2:11][OH:12])[cH:13][nH:14][c:15]12
CCOC(=O)C(N)c1c[nH]c2c(CC)cccc12
CCc1cccc2c(C(N)CO)c[nH]c12
null
null
C1CCOC1
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
c1ccc2[nH]ccc2c1
C-C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[C:3](-[N;D1;H2:4])-[c:5]:[c:6]:[#7;a:7]>>[#7;a:7]:[c:6]:[c:5]-[C:3](-[N;D1;H2:4])-[CH2;D2;+0:1]-[OH;D1;+0:2]
85.7
[{"value": 85.7, "product": "NC(CO)C1=CNC2=C(C=CC=C12)CC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 85.7, "product": "NC(CO)C1=CNC2=C(C=CC=C12)CC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
α-Amino-7-ethyl-1H-indole-3-acetic acid ethyl ester 6 (4.9 g, 0.02 mol) in THF (50 mL) was added to LiAlH4 (2.3 g, 0.06 mol) in THF (25 mL) and the mixture was refluxed for 2 hours to give β-amino-7-ethyl-1H-indole-3-ethanol 7 (3.5 g, 85.7%). A sample recrystallized from ethyl acetate-hexane had m.p. 84°-86° C. Conditi...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
c1ccc2[nH]ccc2c1
HO-
C1CCOC1
null
null
CCOC(=O)C(N)c1c[nH]c2c(CC)cccc12>C1CCOC1>CCc1cccc2c(C(N)CO)c[nH]c12
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-61de906e5c764fd4a50908f805402d9d
CCc1cccc2c3c([nH]c12)C(CC)(CC(=O)OC)OCC3NC=O>>CCc1cccc2c3c([nH]c12)C(CC)(CC(=O)OC)OCC3N
COC(CC1(OCC(C2=C1NC1=C(C=CC=C21)CC)NC=O)CC)=O>>COC(CC1(OCC(C2=C1NC1=C(C=CC=C21)CC)N)CC)=O
O=C[NH:23][CH:22]1[c:8]2[c:7]3[cH:6][cH:5][cH:4][c:3]([CH2:2][CH3:1])[c:11]3[nH:10][c:9]2[C:12]([CH2:13][CH3:14])([CH2:15][C:16](=[O:17])[O:18][CH3:19])[O:20][CH2:21]1>>[CH3:1][CH2:2][c:3]1[cH:4][cH:5][cH:6][c:7]2[c:8]3[c:9]([nH:10][c:11]12)[C:12]([CH2:13][CH3:14])([CH2:15][C:16](=[O:17])[O:18][CH3:19])[O:20][CH2:21][C...
CCc1cccc2c3c([nH]c12)C(CC)(CC(=O)OC)OCC3NC=O
CCc1cccc2c3c([nH]c12)C(CC)(CC(=O)OC)OCC3N
null
null
CO.C
Reduction
Reduction of primary amides to amines
755df58c254dea764fdda078ffd678ec540bba057c83683be04c253f1270ac7b
025f7cefe51e71668ad5d09fca32df168e9b538347403e4d5c1748073e538adc
c1ccc2c3c([nH]c2c1)COCC3
O=C-[NH;D2;+0:1]-[C:2](-[C:3]-[#8:4])-[c:5]:[c:6]:[#7;a:7]>>[#7;a:7]:[c:6]:[c:5]-[C:2](-[NH2;D1;+0:1])-[C:3]-[#8:4]
50
[{"value": 50.0, "product": "COC(CC1(OCC(C2=C1NC1=C(C=CC=C21)CC)N)CC)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 49.9, "product": "COC(CC1(OCC(C2=C1NC1=C(C=CC=C21)CC)N)CC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
1,8-Diethyl-4-formylamino-1,3,4,9-tetrahydropyrano[3,4-b]indole-1-acetic acid methyl ester 10 (5.5 g, 0.01 mol) in 1N methan olic HCl (4.2 mL) and methanol (18 mL) was stirred at 25° C. for 72 hours, then concentrated in vacuo, diluted with water and extracted with ethyl acetate. The aqueous phase was basified with con...
10.6084/m9.figshare.5104873.v1
null
Secondary amide
Primary amine
null
null
c1ccc2c3c([nH]c2c1)COCC3
Other
CO.C
null
null
CCc1cccc2c3c([nH]c12)C(CC)(CC(=O)OC)OCC3NC=O>CO.C>CCc1cccc2c3c([nH]c12)C(CC)(CC(=O)OC)OCC3N
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-5676fe6ae17343b787074a067fa5a00b
CCc1cccc2c3c([nH]c12)C(CC)(CC(=O)OC)OCC3=O>>CCc1cccc2c3c([nH]c12)C(CC)(CC(=O)O)OCC3=O
COC(CC1(OCC(C2=C1NC1=C(C=CC=C21)CC)=O)CC)=O.C(=O)([O-])[O-].[K+].[K+]>>C(C)C1(OCC(C2=C1NC1=C(C=CC=C21)CC)=O)CC(=O)O
C[O:18][C:16]([CH2:15][C:12]1([CH2:13][CH3:14])[c:9]2[c:8]([c:7]3[cH:6][cH:5][cH:4][c:3]([CH2:2][CH3:1])[c:11]3[nH:10]2)[C:21](=[O:22])[CH2:20][O:19]1)=[O:17]>>[CH3:1][CH2:2][c:3]1[cH:4][cH:5][cH:6][c:7]2[c:8]3[c:9]([nH:10][c:11]12)[C:12]([CH2:13][CH3:14])([CH2:15][C:16](=[O:17])[OH:18])[O:19][CH2:20][C:21]3=[O:22]
CCc1cccc2c3c([nH]c12)C(CC)(CC(=O)OC)OCC3=O
CCc1cccc2c3c([nH]c12)C(CC)(CC(=O)O)OCC3=O
null
null
O.CO
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C1COCc2[nH]c3ccccc3c21
C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
93
[{"value": 93.0, "product": "C(C)C1(OCC(C2=C1NC1=C(C=CC=C21)CC)=O)CC(=O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 90.6, "product": "C(C)C1(OCC(C2=C1NC1=C(C=CC=C21)CC)=O)CC(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
1,8-Diethyl-1,3,4,9-tetrahydro-4-oxopyrano[3,4-b]indole-1-acetic acid methyl ester 17 (1.5 g, 4.8 mmol) was suspended in 30 mL of MeOH and a solution of K2CO3 (3.5 g) in 30 mL of H2O was added. The mixture was heated to reflux, upon which the solution became homogeneous. After refluxing for 2 hours, the solution was co...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccc2c3c([nH]c2c1)COCC3
Other
O.CO
null
8
CCc1cccc2c3c([nH]c12)C(CC)(CC(=O)OC)OCC3=O>O.CO>CCc1cccc2c3c([nH]c12)C(CC)(CC(=O)O)OCC3=O
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-a52449461f8f4b61888e8d7e221d8387
C=O.CCC1(CC(=O)OC)OCC(N)c2c1[nH]c1ccccc21>>CCC1(CC(=O)OC)OCC(O)c2c1[nH]c1ccccc21
COC(CC1(OCC(C2=C1NC1=CC=CC=C21)N)CC)=O.O.C=O>>COC(CC1(OCC(C2=C1NC1=CC=CC=C21)O)CC)=O
C=[O:12].N[CH:11]1[CH2:10][O:9][C:3]([CH2:2][CH3:1])([CH2:4][C:5](=[O:6])[O:7][CH3:8])[c:14]2[c:13]1[c:21]1[c:16]([nH:15]2)[cH:17][cH:18][cH:19][cH:20]1>>[CH3:1][CH2:2][C:3]1([CH2:4][C:5](=[O:6])[O:7][CH3:8])[O:9][CH2:10][CH:11]([OH:12])[c:13]2[c:14]1[nH:15][c:16]1[cH:17][cH:18][cH:19][cH:20][c:21]21
C=O.CCC1(CC(=O)OC)OCC(N)c2c1[nH]c1ccccc21
CCC1(CC(=O)OC)OCC(O)c2c1[nH]c1ccccc21
null
null
C1CCOC1
Heteroatom Alkylation and Arylation
OtherReaction
a61cf887c730d83a5dc90e7e80969da43e9c1cb20f0e7096428d2e48ae452b8b
fc7a06eef0b725456f5d7d585d8f3990139808113f032d36dc88ae53908dc6c8
c1ccc2c3c([nH]c2c1)COCC3
C=[O;H0;D1;+0:1].N-[CH;D3;+0:2]1-[C:3]-[#8:4]-[C:5]-[c:6]2:[#7;a:7]:[c:8]:[c:9]:[c:10]:2-1>>[OH;D1;+0:1]-[CH;D3;+0:2]1-[C:3]-[#8:4]-[C:5]-[c:6]2:[#7;a:7]:[c:8]:[c:9]:[c:10]:2-1
66.4
[{"value": 66.4, "product": "COC(CC1(OCC(C2=C1NC1=CC=CC=C21)O)CC)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of 4-amino-1-ethyl-1,3,4,9-tetrahydropyrano[3,4-b]indole-1-acetic acid methyl ester (6 g, 0.020 mol) in 50 mL THF was added 50 mL of H2O and paraformaldehyde (5 g) and the solution was heated at reflux for 2 hours under nitrogen. It was then cooled, concentrated in vacuo, and diluted with ethyl acetate. T...
10.6084/m9.figshare.5104873.v1
null
Formaldehyde.Primary amine
Secondary alcohol
c1ccc2c3c([nH]c2c1)COCC3
c1ccc2c3c([nH]c2c1)COCC3
c1ccc2c3c([nH]c2c1)COCC3
Other
C1CCOC1
null
null
C=O.CCC1(CC(=O)OC)OCC(N)c2c1[nH]c1ccccc21>C1CCOC1>CCC1(CC(=O)OC)OCC(O)c2c1[nH]c1ccccc21
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-3c249d2ea45e4d7eb9c39839b84aa498
CCC1(CC(=O)OC)OCC(O)c2c1[nH]c1ccccc21.[Br][Mg][CH2]c1ccccc1>>CCC1(CC(=O)OC)OCC(Cc2ccccc2)c2c1[nH]c1ccccc21
COC(CC1(OCC(C2=C1NC1=CC=CC=C21)O)CC)=O.C(C1=CC=CC=C1)[Mg]Br>>COC(CC1(OCC(C2=C1NC1=CC=CC=C21)CC2=CC=CC=C2)CC)=O
O[CH:11]1[CH2:10][O:9][C:3]([CH2:2][CH3:1])([CH2:4][C:5](=[O:6])[O:7][CH3:8])[c:20]2[c:19]1[c:27]1[c:22]([nH:21]2)[cH:23][cH:24][cH:25][cH:26]1.[Br][Mg][CH2:12][c:13]1[cH:14][cH:15][cH:16][cH:17][cH:18]1>>[CH3:1][CH2:2][C:3]1([CH2:4][C:5](=[O:6])[O:7][CH3:8])[O:9][CH2:10][CH:11]([CH2:12][c:13]2[cH:14][cH:15][cH:16][cH:...
CCC1(CC(=O)OC)OCC(O)c2c1[nH]c1ccccc21.[Br][Mg][CH2]c1ccccc1
CCC1(CC(=O)OC)OCC(Cc2ccccc2)c2c1[nH]c1ccccc21
null
Cl[Ti](Cl)(Cl)Cl
CCOCC.C(Cl)Cl
C-C Coupling
OtherReaction
55904116283037b89c67502d0ac999187ea061c8887574f4269605b8ffb73765
e5f803b5eba1fcad9c7b7e86e1e67a2a3eda9454e1436fa466e9dc7992ab4bdf
c1ccc(CC2COCc3[nH]c4ccccc4c32)cc1
O-[CH;D3;+0:1]1-[C:2]-[#8:3]-[C:4]-[c:5]2:[#7;a:6]:[c:7]:[c:8]:[c:9]:2-1.[Br]-[Mg]-[CH2;D2;+0:10]-[c:11](:[c:12]):[c:13]>>[c:12]:[c:11](-[CH2;D2;+0:10]-[CH;D3;+0:1]1-[C:2]-[#8:3]-[C:4]-[c:5]2:[#7;a:6]:[c:7]:[c:8]:[c:9]:2-1):[c:13]
51.5
[{"value": 51.5, "product": "COC(CC1(OCC(C2=C1NC1=CC=CC=C21)CC2=CC=CC=C2)CC)=O", "details": "PERCENTYIELD", "is_desired": false}]
-78
CELSIUS
null
null
To a solution of 1-ethyl-4-hydroxy-1,3,4,9-tetrahydropyrano[3,4-b]indole-1-acetic acid methyl ester (1 g, 3.6 mmol) in 60 mL of dry methylene chloride at -78° C. under nitrogen was added TiCl4 in one portion and then after ~10 minutes, a solution of benzyl magnesium bromide in ether was added in one portion and the rea...
10.6084/m9.figshare.5104873.v1
null
Magnesium halide.Secondary alcohol
null
c1ccc2c3c([nH]c2c1)COCC3
c1ccc2c3c([nH]c2c1)COCC3
c1ccccc1.c1ccc2c3c([nH]c2c1)COCC3
HBr.Mg
Cl[Ti](Cl)(Cl)Cl.CCOCC.C(Cl)Cl
-78
null
CCC1(CC(=O)OC)OCC(O)c2c1[nH]c1ccccc21.[Br][Mg][CH2]c1ccccc1>Cl[Ti](Cl)(Cl)Cl.CCOCC.C(Cl)Cl>CCC1(CC(=O)OC)OCC(Cc2ccccc2)c2c1[nH]c1ccccc21
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-9556cefffb024358a20dc4af2da2b613
CCC1(CC(=O)OC)OCC(Cc2ccccc2)c2c1[nH]c1ccccc21>>CCC1(CC(=O)O)OCC(Cc2ccccc2)c2c1[nH]c1ccccc21
COC(CC1(OCC(C2=C1NC1=CC=CC=C21)CC2=CC=CC=C2)CC)=O.[OH-].[Na+]>>C(C1=CC=CC=C1)C1COC(C=2NC3=CC=CC=C3C21)(CC(=O)O)CC
C[O:7][C:5]([CH2:4][C:3]1([CH2:2][CH3:1])[O:8][CH2:9][CH:10]([CH2:11][c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[c:18]2[c:19]1[nH:20][c:21]1[cH:22][cH:23][cH:24][cH:25][c:26]21)=[O:6]>>[CH3:1][CH2:2][C:3]1([CH2:4][C:5](=[O:6])[OH:7])[O:8][CH2:9][CH:10]([CH2:11][c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[c:18]2[c:19]1...
CCC1(CC(=O)OC)OCC(Cc2ccccc2)c2c1[nH]c1ccccc21
CCC1(CC(=O)O)OCC(Cc2ccccc2)c2c1[nH]c1ccccc21
null
null
C(C)O
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(CC2COCc3[nH]c4ccccc4c32)cc1
C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
82
[{"value": 80.0, "product": "C(C1=CC=CC=C1)C1COC(C=2NC3=CC=CC=C3C21)(CC(=O)O)CC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 82.0, "product": "C(C1=CC=CC=C1)C1COC(C=2NC3=CC=CC=C3C21)(CC(=O)O)CC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of 4-benzyl-1-ethyl-1,3,4,9-tetrahydropyrano[3,4-b]indole-1-acetic acid methyl ester (0.67 g, 1.8 mmol) in 30 mL of ethanol was added 30 mL of 10% solution of sodium hydroxide and heated at reflux for 2 hours under nitrogen. The reaction mixture was then cooled and concentrated in vacuo, diluted with 20 m...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccc2c3c([nH]c2c1)COCC3
Other
C(C)O
null
null
CCC1(CC(=O)OC)OCC(Cc2ccccc2)c2c1[nH]c1ccccc21>C(C)O>CCC1(CC(=O)O)OCC(Cc2ccccc2)c2c1[nH]c1ccccc21
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-01fa6ac283af4ba48f163633f0be11dd
CCOC(=O)c1ncc[nH]1.O=[N+]([O-])c1ccccc1CCl>>CCOC(=O)c1nccn1Cc1ccccc1[N+](=O)[O-]
N1C(=NC=C1)C(=O)OCC.[N+](=O)([O-])C1=C(CCl)C=CC=C1.C([O-])([O-])=O.[K+].[K+]>>[N+](=O)([O-])C1=C(CN2C(=NC=C2)C(=O)OCC)C=CC=C1
[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[n:7][cH:8][cH:9][nH:10]1.Cl[CH2:11][c:12]1[cH:13][cH:14][cH:15][cH:16][c:17]1[N+:18](=[O:19])[O-:20]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[n:7][cH:8][cH:9][n:10]1[CH2:11][c:12]1[cH:13][cH:14][cH:15][cH:16][c:17]1[N+:18](=[O:19])[O-:20]
CCOC(=O)c1ncc[nH]1.O=[N+]([O-])c1ccccc1CCl
CCOC(=O)c1nccn1Cc1ccccc1[N+](=O)[O-]
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
5118ce9eea46859cccf16d01cf8151757afd816de0c93fe6fcb74a0ee15c5a67
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ccc(Cn2ccnc2)cc1
Cl-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[C:5]-[#8:6]-[C:7](=[O;D1;H0:8])-[c:9]1:[#7;a:10]:[c:11]:[c:12]:[nH;D2;+0:13]:1>>[C:5]-[#8:6]-[C:7](=[O;D1;H0:8])-[c:9]1:[#7;a:10]:[c:11]:[c:12]:[n;H0;D3;+0:13]:1-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
85.4
[{"value": 85.4, "product": "[N+](=O)([O-])C1=C(CN2C(=NC=C2)C(=O)OCC)C=CC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 85.4, "product": "[N+](=O)([O-])C1=C(CN2C(=NC=C2)C(=O)OCC)C=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
null
null
A mixture of 14 g (0.1 mol) of ethyl imidazol-2-carboxylate, 18.9 g (0.11 mol) of o-nitrobenzyl chloride, 13.8 g (0.1 mol) of anhydrous potassium carbonate and 100 ml of dimethylformamide was heated at 100° C. for 2 hours while stirring. Then, the solvent was substantially distilled off in vacuo, the residue was mixed ...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1c[nH]cn1
c1ncc[nH]1
c1ncc[nH]1.c1ccccc1
HCl
CN(C=O)C
100
null
CCOC(=O)c1ncc[nH]1.O=[N+]([O-])c1ccccc1CCl>CN(C=O)C>CCOC(=O)c1nccn1Cc1ccccc1[N+](=O)[O-]
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-1127223cbea3488e85342ef665537ecd
CCOC(=O)c1nccn1Cc1ccccc1[N+](=O)[O-]>>CCOC(=O)c1nccn1Cc1ccccc1N
[N+](=O)([O-])C1=C(CN2C(=NC=C2)C(=O)OCC)C=CC=C1>>NC1=C(CN2C(=NC=C2)C(=O)OCC)C=CC=C1
O=[N+:18]([O-])[c:17]1[c:12]([CH2:11][n:10]2[c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[n:7][cH:8][cH:9]2)[cH:13][cH:14][cH:15][cH:16]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[n:7][cH:8][cH:9][n:10]1[CH2:11][c:12]1[cH:13][cH:14][cH:15][cH:16][c:17]1[NH2:18]
CCOC(=O)c1nccn1Cc1ccccc1[N+](=O)[O-]
CCOC(=O)c1nccn1Cc1ccccc1N
null
[Ni]
O1CCCC1
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc(Cn2ccnc2)cc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
85.4
[{"value": 85.4, "product": "NC1=C(CN2C(=NC=C2)C(=O)OCC)C=CC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 85.4, "product": "NC1=C(CN2C(=NC=C2)C(=O)OCC)C=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
49.6 g (0.18 mol) of ethyl 1-(2-nitrobenzyl)-imidazole-2-carboxylate were hydrogenated in 500 ml of tetrahydrofuran at room temperature under a pressure of 5 bar in the presence of Raney nickel. After the theoretical quantity of hydrogen had been absorbed, the catalyst was suction-filtered off, and the filtrate was eva...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ncc[nH]1.c1ccccc1
Other
[Ni].O1CCCC1
null
null
CCOC(=O)c1nccn1Cc1ccccc1[N+](=O)[O-]>[Ni].O1CCCC1>CCOC(=O)c1nccn1Cc1ccccc1N
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-938dad52bf424847b5a87b0af4a64a9c
CCCCCCCCCCCCCCCCCCN.O=C[C@H](O)[C@@H](O)[C@H](O)[C@H](O)CO>>CCCCCCCCCCCCCCCCCCNC1O[C@H](CO)[C@@H](O)[C@H](O)[C@H]1O
C(CCCCCCCCCCCCCCCCC)N.O=C[C@H](O)[C@@H](O)[C@H](O)[C@H](O)CO>>C(CCCCCCCCCCCCCCCCC)NC1[C@H](O)[C@@H](O)[C@H](O)[C@H](O1)CO
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][CH2:13][CH2:14][CH2:15][CH2:16][CH2:17][CH2:18][NH2:19].O=[CH:20][C@H:22]([OH:21])[C@@H:25]([OH:26])[C@H:27]([OH:28])[C@@H:29]([CH2:23][OH:24])[OH:30]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][...
CCCCCCCCCCCCCCCCCCN.O=C[C@H](O)[C@@H](O)[C@H](O)[C@H](O)CO
CCCCCCCCCCCCCCCCCCNC1O[C@H](CO)[C@@H](O)[C@H](O)[C@H]1O
null
null
C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
700d99fb45e8c08897a966fba4f347880bc47ef6e630efe8f099c330952bc13f
7b4a51bec8d1f2dbd10dc44a9694073db624a60f2ad010a97db84ae5bad43264
C1CCOCC1
O=[CH;D2;+0:1]-[C@H;D3;+0:2](-[OH;D1;+0:3])-[C:4](-[O;D1;H1:5])-[C:6](-[O;D1;H1:7])-[C@H;D3;+0:8](-[O;D1;H1:9])-[CH2;D2;+0:10]-[O;D1;H1:11].[C:12]-[C:13]-[NH2;D1;+0:14]>>[C:12]-[C:13]-[NH;D2;+0:14]-[CH;D3;+0:1]1-[O;H0;D2;+0:3]-[C@H;D3;+0:2](-[CH2;D2;+0:10]-[O;D1;H1:11])-[C:4](-[O;D1;H1:5])-[C:6](-[O;D1;H1:7])-[C@H;D3;+...
null
[]
70
CELSIUS
15
MINUTE
20 g of octadecylamine are dissolved in 120 ml of ethanol and the solution is warmed to 70° C. 11 g of anhydrous D-glucose are added. After a clear solution has formed, stirring is continued at 70° C. for a further 15 minutes. The solution is cooled to 10° C. and left to stand for 15 minutes. The crystal sludge formed ...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary alcohol.Secondary alcohol.Secondary alcohol.Primary amine
Ether.Primary alcohol.Secondary alcohol.Secondary amine
null
C1CCOCC1
C1CCOCC1
HO-
C(C)O
70
0.25
CCCCCCCCCCCCCCCCCCN.O=C[C@H](O)[C@@H](O)[C@H](O)[C@H](O)CO>C(C)O>CCCCCCCCCCCCCCCCCCNC1O[C@H](CO)[C@@H](O)[C@H](O)[C@H]1O
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-e81b667d9aad48d78623dcbfce1d50b3
CCCCCCCCCCCCN.O=C[C@@H](O)[C@@H](O)[C@H](O)CO>>CCCCCCCCCCCCN(C(=O)CCCCCCCCCCC)C1OC[C@@H](O)[C@H](O)[C@@H]1O
O=C[C@@H](O)[C@@H](O)[C@H](O)CO.O.C(CCCCCCCCCCC)N>>C1([C@@H](O)[C@@H](O)[C@H](O)CO1)N(C(CCCCCCCCCCC)=O)CCCCCCCCCCCC
[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][NH2:13].[CH:14](=[O:15])[C@H:16]([C@H:17]([C@@H:18]([CH2:29][OH:28])[OH:33])[OH:35])[OH:31]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][N:13]([C:14](=[O:15])[CH2:16][CH2:17][CH2:18][CH2:1...
CCCCCCCCCCCCN.O=C[C@@H](O)[C@@H](O)[C@H](O)CO
CCCCCCCCCCCCN(C(=O)CCCCCCCCCCC)C1OC[C@@H](O)[C@H](O)[C@@H]1O
null
null
C(C)(C)O
Acylation
OtherReaction
bd12222f5a1dbc90ca4ad198aa569e19fc1d179bf399e9bbb35041bb97e6d0ae
9f2b424da96061e4cbc2dc7b3a873dbb8a3ff62181cbd30d1d5a49c911995492
C1CCOCC1
[C:1]-[C:2]-[NH2;D1;+0:3].[O;D1;H0:4]=[CH;D2;+0:5]-[C@@H;D3;+0:6](-[OH;D1;+0:7])-[C@@H;D3;+0:8](-[OH;D1;+0:9])-[C@H;D3;+0:10](-[OH;D1;+0:11])-[CH2;D2;+0:12]-[OH;D1;+0:13]>>[C:1]-[C:2]-[N;H0;D3;+0:3](-[C:14]1-[O;H0;D2;+0:13]-[CH2;D2;+0:12]-[C:15](-[OH;D1;+0:7])-[C:16](-[OH;D1;+0:11])-[C:17]-1-[OH;D1;+0:9])-[C;H0;D3;+0:5...
null
[]
null
null
null
null
10 g of D-lyxose are dissolved in 120 ml of isopropanol and 60 ml of water and the solution is warmed to 70° C. 18 g of dodecylamine are added. After a clear solution has formed, the temperature is maintained for a further 15 minutes. The mixture is cooled to room temperature and evaporated in vacuo. 10 g of the result...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary alcohol.Secondary alcohol.Secondary alcohol.Secondary alcohol.Primary amine
Ether.Tertiary amide.Secondary alcohol.Secondary alcohol.Secondary alcohol
null
C1CCOCC1
C1CCOCC1
Other
C(C)(C)O
null
null
CCCCCCCCCCCCN.O=C[C@@H](O)[C@@H](O)[C@H](O)CO>C(C)(C)O>CCCCCCCCCCCCN(C(=O)CCCCCCCCCCC)C1OC[C@@H](O)[C@H](O)[C@@H]1O
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-c0f934309e2b409e80e6ac307eb62b54
CC12OC1C(=O)c1ccccc1C2=O>>CC1=CC(=O)c2ccccc2C1=O
O1C2(C(C3=CC=CC=C3C(C21)=O)=O)C>>CC1=CC(C2=CC=CC=C2C1=O)=O
O1[C:2]2([CH3:1])[CH:3]1[C:4](=[O:5])[c:6]1[cH:7][cH:8][cH:9][cH:10][c:11]1[C:12]2=[O:13]>>[CH3:1][C:2]1=[CH:3][C:4](=[O:5])[c:6]2[cH:7][cH:8][cH:9][cH:10][c:11]2[C:12]1=[O:13]
CC12OC1C(=O)c1ccccc1C2=O
CC1=CC(=O)c2ccccc2C1=O
null
null
C(C)O
Miscellaneous
OtherReaction
d9329f4b756907c222746c94c6a03d3126b49c1318996b5c6b83c4aa3a1d40af
4332fe0ec601bde18c21b5783b9089cdaa378b1cc06a7c680f8caa518ecaad9e
O=C1C=CC(=O)c2ccccc21
[C;D1;H3:1]-[C;H0;D4;+0:2]12-O-[CH;D3;+0:3]-1-[C:4](=[O;D1;H0:5])-[c:6]:[c:7]-[C:8]-2=[O;D1;H0:9]>>[C;D1;H3:1]-[C;H0;D3;+0:2]1=[CH;D2;+0:3]-[C:4](=[O;D1;H0:5])-[c:6]:[c:7]-[C:8]-1=[O;D1;H0:9]
null
[]
null
null
null
null
According to Flowchart V, 2,3-epoxy-2-methyl-1,4-naphthoquinone 11 is reacted with an amine 2, where R2, R3, R4 and R5 are as described above, in absolute ethanol with heat for several hours, producing the 3-methyl-1,4-naphthalenedione derivatives 12. Conditions: See reaction.notes.procedure_details. Workup: with heat ...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ketone.Ether
Ketone.Ketone
c1ccc2c(c1)CC1OC1C2
C1=CCc2ccccc2C1
C1=CCc2ccccc2C1
Other
C(C)O
null
null
CC12OC1C(=O)c1ccccc1C2=O>C(C)O>CC1=CC(=O)c2ccccc2C1=O
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-5e5ab1b93bec4eba8877cca84ee8b3fb
CCOC(=O)N1CCNCC1.O=C1C(Cl)=C(Cl)C(=O)c2ccccc21>>CCOC(=O)N1CCN(C2=C(Cl)C(=O)c3ccccc3C2=O)CC1
ClC=1C(C2=CC=CC=C2C(C1Cl)=O)=O.N1(CCNCC1)C(=O)OCC>>ClC1=C(C(C2=CC=CC=C2C1=O)=O)N1CCN(CC1)C(=O)OCC
[CH3:1][CH2:2][O:3][C:4](=[O:5])[N:6]1[CH2:7][CH2:8][NH:9][CH2:23][CH2:24]1.Cl[C:10]1=[C:11]([Cl:12])[C:13](=[O:14])[c:15]2[cH:16][cH:17][cH:18][cH:19][c:20]2[C:21]1=[O:22]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[N:6]1[CH2:7][CH2:8][N:9]([C:10]2=[C:11]([Cl:12])[C:13](=[O:14])[c:15]3[cH:16][cH:17][cH:18][cH:19][c:20]3[C:21]2=...
CCOC(=O)N1CCNCC1.O=C1C(Cl)=C(Cl)C(=O)c2ccccc21
CCOC(=O)N1CCN(C2=C(Cl)C(=O)c3ccccc3C2=O)CC1
null
null
C(C)O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
0912e26e7d1eb0222158d18478bb8682658ea8b99a047d9cfd5ddf1ce0ba8013
933b337e66ad3bf71c4790533c0d1ebcae3a16ae4bb9f3b59c4a11d8d3c64228
O=C1C=C(N2CCNCC2)C(=O)c2ccccc21
Cl-[C;H0;D3;+0:1]1=[C:2](-[Cl;D1;H0:3])-[C:4](=[O;D1;H0:5])-[c:6]:[c:7]-[C:8]-1=[O;D1;H0:9].[#7:10]1-[C:11]-[C:12]-[NH;D2;+0:13]-[C:14]-[C:15]-1>>[Cl;D1;H0:3]-[C:2]1=[C;H0;D3;+0:1](-[N;H0;D3;+0:13]2-[C:12]-[C:11]-[#7:10]-[C:15]-[C:14]-2)-[C:8](=[O;D1;H0:9])-[c:7]:[c:6]-[C:4]-1=[O;D1;H0:5]
45.9
[{"value": 45.9, "product": "ClC1=C(C(C2=CC=CC=C2C1=O)=O)N1CCN(CC1)C(=O)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 11.35 g of 2,3-dichloro-1,4-naphthoquinone, 15.8 g of 1-piperazinecarboxylic acid, ethyl ester and 400 ml of absolute ethanol was heated at reflux for 3 hours and then evaporated to dryness. The residue was taken up in 300 ml of dichloromethane and filtered through silica gel. The filtrate was evaporated a...
10.6084/m9.figshare.5104873.v1
null
Alkenyl halide.Ketone.Secondary amine
Enamine
C1C[NH]CCN1.C1=CCc2ccccc2C1
C1C[NH]CC[NH]1.C1=CCc2ccccc2C1
C1C[NH]CC[NH]1.C1=CCc2ccccc2C1
HCl
C(C)O
null
null
CCOC(=O)N1CCNCC1.O=C1C(Cl)=C(Cl)C(=O)c2ccccc21>C(C)O>CCOC(=O)N1CCN(C2=C(Cl)C(=O)c3ccccc3C2=O)CC1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-1eafa52968e943938f9fb0c465258a6f
CNCCN(C)Cc1ccccc1.O=C1C(Cl)=C(Cl)C(=O)c2ccccc21>>CN(CCN(C)C1=C(Cl)C(=O)c2ccccc2C1=O)Cc1ccccc1.Cl
CNCCN(CC1=CC=CC=C1)C.ClC=1C(C2=CC=CC=C2C(C1Cl)=O)=O>>Cl.ClC=1C(C2=CC=CC=C2C(C1N(CCN(CC1=CC=CC=C1)C)C)=O)=O
[CH3:1][N:2]([CH2:3][CH2:4][NH:5][CH3:6])[CH2:20][c:21]1[cH:22][cH:23][cH:24][cH:25][cH:26]1.[C:7]1([Cl:27])=[C:8]([Cl:9])[C:10](=[O:11])[c:12]2[cH:13][cH:14][cH:15][cH:16][c:17]2[C:18]1=[O:19]>>[CH3:1][N:2]([CH2:3][CH2:4][N:5]([CH3:6])[C:7]1=[C:8]([Cl:9])[C:10](=[O:11])[c:12]2[cH:13][cH:14][cH:15][cH:16][c:17]2[C:18]1...
CNCCN(C)Cc1ccccc1.O=C1C(Cl)=C(Cl)C(=O)c2ccccc21
CN(CCN(C)C1=C(Cl)C(=O)c2ccccc2C1=O)Cc1ccccc1.Cl
null
null
C(C)O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
6f37a459d2fb11a17a9e97f5cd042e976fec1a8ec93175c8f9dea954d9e1125b
d366d1b6aa9b6e9510093ba8fd2f2edd66587096816415e691b2ed113a22fc6c
O=C1C=C(NCCNCc2ccccc2)C(=O)c2ccccc21
[C:1]-[C:2]-[NH;D2;+0:3]-[C;D1;H3:4].[Cl;D1;H0:5]-[C:6]1=[C;H0;D3;+0:7](-[Cl;H0;D1;+0:8])-[C:9](=[O;D1;H0:10])-[c:11]:[c:12]-[C:13]-1=[O;D1;H0:14]>>[C:1]-[C:2]-[N;H0;D3;+0:3](-[C;D1;H3:4])-[C;H0;D3;+0:7]1=[C:6](-[Cl;D1;H0:5])-[C:13](=[O;D1;H0:14])-[c:12]:[c:11]-[C:9]-1=[O;D1;H0:10].[ClH;D0;+0:8]
null
[]
-10
CELSIUS
16
HOUR
A 4.5 g portion of methyl 2-[methyl(phenylmethyl)amino]ethylamine was added to a stirred slurry of 5.6 g of 2,3-dichloro-1,4-naphthoquinone in 150 ml of absolute ethanol. Stirring was continued for 16 hours, then the mixture was heated at reflux for one hour and filtered while hot. The mixture was then cooled at -10° C...
10.6084/m9.figshare.5104873.v1
null
Alkenyl halide.Ketone.Secondary amine
Enamine.Ketone
C1=CCc2ccccc2C1
C1=CCc2ccccc2C1
C1=CCc2ccccc2C1.c1ccccc1
null
C(C)O
-10
16
CNCCN(C)Cc1ccccc1.O=C1C(Cl)=C(Cl)C(=O)c2ccccc21>C(C)O>CN(CCN(C)C1=C(Cl)C(=O)c2ccccc2C1=O)Cc1ccccc1.Cl
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-bbb9c2f74808455388a035da8c8a3eeb
CC(=O)NC1=C(Cl)C(=O)c2ccccc2C1=O.c1ccc(CN2CCNCC2)cc1>>CC(=O)NC1=C(N2CCN(Cc3ccccc3)CC2)C(=O)c2ccccc2C1=O
C(C)(=O)NC=1C(C2=CC=CC=C2C(C1Cl)=O)=O.C(C1=CC=CC=C1)N1CCNCC1>>O=C1C(=C(C(C2=CC=CC=C12)=O)N1CCN(CC1)CC1=CC=CC=C1)NC(C)=O
Cl[C:6]1=[C:5]([NH:4][C:2]([CH3:1])=[O:3])[C:28](=[O:29])[c:27]2[c:22]([cH:23][cH:24][cH:25][cH:26]2)[C:20]1=[O:21].[NH:7]1[CH2:8][CH2:9][N:10]([CH2:11][c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[CH2:18][CH2:19]1>>[CH3:1][C:2](=[O:3])[NH:4][C:5]1=[C:6]([N:7]2[CH2:8][CH2:9][N:10]([CH2:11][c:12]3[cH:13][cH:14][cH:15][cH...
CC(=O)NC1=C(Cl)C(=O)c2ccccc2C1=O.c1ccc(CN2CCNCC2)cc1
CC(=O)NC1=C(N2CCN(Cc3ccccc3)CC2)C(=O)c2ccccc2C1=O
null
null
C(C)O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
d4a0d8c63c5bbf8e6b2a19dd3b1761c1fda17365ba7c27585f8e97bb31c6dca1
2f1af1bc2b6a104816ee6e304bb76145e9e36ef858bc716179b7b9df9c8858ef
O=C1C=C(N2CCN(Cc3ccccc3)CC2)C(=O)c2ccccc21
Cl-[C;H0;D3;+0:1]1=[C:2](-[#7:3]-[C:4](-[C;D1;H3:5])=[O;D1;H0:6])-[C:7](=[O;D1;H0:8])-[c:9]:[c:10]-[C:11]-1=[O;D1;H0:12].[#7:13]1-[C:14]-[C:15]-[NH;D2;+0:16]-[C:17]-[C:18]-1>>[C;D1;H3:5]-[C:4](=[O;D1;H0:6])-[#7:3]-[C:2]1=[C;H0;D3;+0:1](-[N;H0;D3;+0:16]2-[C:15]-[C:14]-[#7:13]-[C:18]-[C:17]-2)-[C:11](=[O;D1;H0:12])-[c:10...
89.7
[{"value": 89.7, "product": "O=C1C(=C(C(C2=CC=CC=C12)=O)N1CCN(CC1)CC1=CC=CC=C1)NC(C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 500 mg of 2-acetylamino-3-chloro-1,4-naphthoquinone, 880 mg of N-benzylpiperazine and 40 ml of absolute ethanol was heated at reflux for 3 hours, then the solvent was removed. The remainder was passed through a small plug of silica gel and eluted with chloroform. The eluate was concentrated to a solid whic...
10.6084/m9.figshare.5104873.v1
null
Enamine.Alkenyl halide.Ketone.Secondary amine
Enamine.Enamine
C1=CCc2ccccc2C1.C1CNCC[NH]1
C1C[NH]CC[NH]1.C1=CCc2ccccc2C1
C1C[NH]CC[NH]1.c1ccccc1.C1=CCc2ccccc2C1
HCl
C(C)O
null
null
CC(=O)NC1=C(Cl)C(=O)c2ccccc2C1=O.c1ccc(CN2CCNCC2)cc1>C(C)O>CC(=O)NC1=C(N2CCN(Cc3ccccc3)CC2)C(=O)c2ccccc2C1=O
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-da7582724371467fa51419dee56b16ee
CCCCOC(=O)Cl.O=C1C(Cl)=C(N2CCNCC2)C(=O)c2ccccc21>>CC(C)COC(=O)N1CCN(C2=C(Cl)C(=O)c3ccccc3C2=O)CC1
ClC1=C(C(C2=CC=CC=C2C1=O)=O)N1CCNCC1.ClC(=O)OCCCC.O1CCCC1.O1CCCC1>>ClC1=C(C(C2=CC=CC=C2C1=O)=O)N1CCN(CC1)C(=O)OCC(C)C
Cl[C:6]([O:5][CH2:4][CH2:2][CH2:1][CH3:3])=[O:7].[NH:8]1[CH2:9][CH2:10][N:11]([C:12]2=[C:13]([Cl:14])[C:15](=[O:16])[c:17]3[cH:18][cH:19][cH:20][cH:21][c:22]3[C:23]2=[O:24])[CH2:25][CH2:26]1>>[CH3:1][CH:2]([CH3:3])[CH2:4][O:5][C:6](=[O:7])[N:8]1[CH2:9][CH2:10][N:11]([C:12]2=[C:13]([Cl:14])[C:15](=[O:16])[c:17]3[cH:18][...
CCCCOC(=O)Cl.O=C1C(Cl)=C(N2CCNCC2)C(=O)c2ccccc21
CC(C)COC(=O)N1CCN(C2=C(Cl)C(=O)c3ccccc3C2=O)CC1
null
null
null
C-C Coupling
OtherReaction
09de75b17c7eee1289e3b190226d6ad52495b2ae0a16b9cd4889f920cc52f2c2
af3aa3e2f147b2df60916d28a16c97cabb605429e921245c8b8e12ed2ec35188
O=C1C=C(N2CCNCC2)C(=O)c2ccccc21
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C:4]-[CH2;D2;+0:5]-[CH2;D2;+0:6]-[CH3;D1;+0:7].[#7:8]1-[C:9]-[C:10]-[NH;D2;+0:11]-[C:12]-[C:13]-1>>[CH3;D1;+0:6]-[CH;D3;+0:5](-[CH3;D1;+0:7])-[C:4]-[#8:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[N;H0;D3;+0:11]1-[C:12]-[C:13]-[#7:8]-[C:9]-[C:10]-1
null
[]
null
null
20
MINUTE
A solution of 830 mg of 3-chloro-2-piperazinyl-1,4-naphthoquinone in 50 ml of tetrahydrofuran was added dropwise to a solution of 0.39 ml of butyl chloroformate in 10 ml of tetrahydrofuran. This mixture was stirred for 20 minutes, then filtered and the filtrate concentrated to an oil. The oil was recrystallized from et...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Ether.Secondary amine
Carbamic ester.Ether
C1CNCC[NH]1
C1C[NH]CC[NH]1
C1C[NH]CC[NH]1.C1=CCc2ccccc2C1
HCl
null
null
0.333333
CCCCOC(=O)Cl.O=C1C(Cl)=C(N2CCNCC2)C(=O)c2ccccc21>>CC(C)COC(=O)N1CCN(C2=C(Cl)C(=O)c3ccccc3C2=O)CC1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-bd93f5c31e3a4d1182f4de13828044bc
CC12OC1C(=O)c1ccccc1C2=O.CCOC(=O)N1CCNCC1>>CCOC(=O)N1CCN(C2=C(C)C(=O)c3ccccc3C2=O)CC1
O1C2C(C3=CC=CC=C3C(C21C)=O)=O.N1(CCNCC1)C(=O)OCC>>CC1=C(C(C2=CC=CC=C2C1=O)=O)N1CCN(CC1)C(=O)OCC
O1[CH:10]2[C:11]1([CH3:12])[C:13](=[O:14])[c:15]1[cH:16][cH:17][cH:18][cH:19][c:20]1[C:21]2=[O:22].[CH3:1][CH2:2][O:3][C:4](=[O:5])[N:6]1[CH2:7][CH2:8][NH:9][CH2:23][CH2:24]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[N:6]1[CH2:7][CH2:8][N:9]([C:10]2=[C:11]([CH3:12])[C:13](=[O:14])[c:15]3[cH:16][cH:17][cH:18][cH:19][c:20]3[C:21...
CC12OC1C(=O)c1ccccc1C2=O.CCOC(=O)N1CCNCC1
CCOC(=O)N1CCN(C2=C(C)C(=O)c3ccccc3C2=O)CC1
null
null
C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
c7d49f3b46b25ba8d4f47861ba897f9b2a406154c4f8af99f3731b072bf67e93
85d3530ea2ab12eabae6f8a679c30f9a97b0d5a6a810726450a36f9da54ec15c
O=C1C=C(N2CCNCC2)C(=O)c2ccccc21
[#7:1]1-[C:2]-[C:3]-[NH;D2;+0:4]-[C:5]-[C:6]-1.[C;D1;H3:7]-[C;H0;D4;+0:8]12-O-[CH;D3;+0:9]-1-[C:10](=[O;D1;H0:11])-[c:12]:[c:13]-[C:14]-2=[O;D1;H0:15]>>[C;D1;H3:7]-[C;H0;D3;+0:8]1=[C;H0;D3;+0:9](-[N;H0;D3;+0:4]2-[C:3]-[C:2]-[#7:1]-[C:6]-[C:5]-2)-[C:10](=[O;D1;H0:11])-[c:12]:[c:13]-[C:14]-1=[O;D1;H0:15]
30.5
[{"value": 30.5, "product": "CC1=C(C(C2=CC=CC=C2C1=O)=O)N1CCN(CC1)C(=O)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
50
CELSIUS
12
HOUR
A mixture of 1.88 g of 2,3-epoxy-3-methyl-1,4-naphthoquinone, 3.16 g of piperazinecarboxylic acid, ethyl ester and 100 ml of absolute ethanol was stirred for 12 hours at 50° C. The solvent was then removed and the remainder filtered through a one inch plug of silica gel and eluted with chloroform. The eluate was evapor...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ketone.Ether.Secondary amine
Enamine
c1ccc2c(c1)CC1OC1C2.C1C[NH]CCN1
C1C[NH]CC[NH]1.C1=CCc2ccccc2C1
C1C[NH]CC[NH]1.C1=CCc2ccccc2C1
HO-
C(C)O
50
12
CC12OC1C(=O)c1ccccc1C2=O.CCOC(=O)N1CCNCC1>C(C)O>CCOC(=O)N1CCN(C2=C(C)C(=O)c3ccccc3C2=O)CC1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-9932b54276624110a863e2acdaabdbe2
CC1=C(N2CCNCC2)C(=O)c2ccccc2C1=O.O=C=Nc1ccc(Cl)cc1>>CC1=C(N2CCN(C(=O)Nc3ccc(Cl)cc3)CC2)C(=O)c2ccccc2C1=O
CC1=C(C(C2=CC=CC=C2C1=O)=O)N1CCNCC1.ClC1=CC=C(C=C1)N=C=O>>ClC1=CC=C(C=C1)NC(=O)N1CCN(CC1)C=1C(C2=CC=CC=C2C(C1C)=O)=O
[CH3:1][C:2]1=[C:3]([N:4]2[CH2:5][CH2:6][NH:7][CH2:18][CH2:19]2)[C:20](=[O:21])[c:22]2[cH:23][cH:24][cH:25][cH:26][c:27]2[C:28]1=[O:29].[C:8](=[O:9])=[N:10][c:11]1[cH:12][cH:13][c:14]([Cl:15])[cH:16][cH:17]1>>[CH3:1][C:2]1=[C:3]([N:4]2[CH2:5][CH2:6][N:7]([C:8](=[O:9])[NH:10][c:11]3[cH:12][cH:13][c:14]([Cl:15])[cH:16][c...
CC1=C(N2CCNCC2)C(=O)c2ccccc2C1=O.O=C=Nc1ccc(Cl)cc1
CC1=C(N2CCN(C(=O)Nc3ccc(Cl)cc3)CC2)C(=O)c2ccccc2C1=O
null
null
O1CCCC1
Acylation
Urea synthesis via isocyanate and secondary amine
6fdae4b903e981d8b7a376762a2f4ccd0c6fe7e77f0529898c101f9e9062d1aa
5272a383a93723269f1934f97993b0175b43cd993bcdf2f45add1dbb852d1e09
O=C1C=C(N2CCN(C(=O)Nc3ccccc3)CC2)C(=O)c2ccccc21
[#7:1]1-[C:2]-[C:3]-[NH;D2;+0:4]-[C:5]-[C:6]-1.[O;D1;H0:7]=[C;H0;D2;+0:8]=[N;H0;D2;+0:9]-[c:10](:[c:11]):[c:12]>>[O;D1;H0:7]=[C;H0;D3;+0:8](-[NH;D2;+0:9]-[c:10](:[c:11]):[c:12])-[N;H0;D3;+0:4]1-[C:3]-[C:2]-[#7:1]-[C:6]-[C:5]-1
83.4
[{"value": 83.4, "product": "ClC1=CC=C(C=C1)NC(=O)N1CCN(CC1)C=1C(C2=CC=CC=C2C(C1C)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
0.5
HOUR
A solution of 150 mg of 3-methyl-2-piperazinyl-1,4-naphthoquinone in 50 ml of tetrahydrofuran was treated with a solution of 100 mg of 4-chlorophenylisocyanate in 10 ml of tetrahydrofuran. This mixture was stirred 1/2 hour, then evaporated in vacuo and the residue taken up in dichloromethane and filtered. The filtrate ...
10.6084/m9.figshare.5104873.v1
null
Isocyanate.Secondary amine
Urea
C1C[NH]CCN1
C1C[NH]CC[NH]1
C1C[NH]CC[NH]1.c1ccccc1.C1=CCc2ccccc2C1
null
O1CCCC1
null
0.5
CC1=C(N2CCNCC2)C(=O)c2ccccc2C1=O.O=C=Nc1ccc(Cl)cc1>O1CCCC1>CC1=C(N2CCN(C(=O)Nc3ccc(Cl)cc3)CC2)C(=O)c2ccccc2C1=O
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-e28d3533b1644cf894614640d3f6f843
O=C1C(Cl)=C(N2CCNCC2)C(=O)c2ccccc21.O=S(=O)(Cl)c1ccccc1C(F)(F)F>>O=C1C(Cl)=C(N2CCN(S(=O)(=O)c3ccccc3C(F)(F)F)CC2)C(=O)c2ccccc21
ClC1=C(C(C2=CC=CC=C2C1=O)=O)N1CCNCC1.FC(C1=C(C=CC=C1)S(=O)(=O)Cl)(F)F>>ClC1=C(C(C2=CC=CC=C2C1=O)=O)N1CCN(CC1)S(=O)(=O)C1=C(C=CC=C1)C(F)(F)F
[O:1]=[C:2]1[C:3]([Cl:4])=[C:5]([N:6]2[CH2:7][CH2:8][NH:9][CH2:23][CH2:24]2)[C:25](=[O:26])[c:27]2[cH:28][cH:29][cH:30][cH:31][c:32]21.Cl[S:10](=[O:11])(=[O:12])[c:13]1[cH:14][cH:15][cH:16][cH:17][c:18]1[C:19]([F:20])([F:21])[F:22]>>[O:1]=[C:2]1[C:3]([Cl:4])=[C:5]([N:6]2[CH2:7][CH2:8][N:9]([S:10](=[O:11])(=[O:12])[c:13...
O=C1C(Cl)=C(N2CCNCC2)C(=O)c2ccccc21.O=S(=O)(Cl)c1ccccc1C(F)(F)F
O=C1C(Cl)=C(N2CCN(S(=O)(=O)c3ccccc3C(F)(F)F)CC2)C(=O)c2ccccc21
null
null
null
Acylation
Sulfonamide synthesis (Schotten-Baumann) secondary amine
c6a995ab9be6571957febbe378833244177e30fd671e64e4e1ffe6f50345cf56
b7aca5a5d690b0846685a854bc946849e1041bfc3965161290b5ffb2821af09e
O=C1C=C(N2CCN(S(=O)(=O)c3ccccc3)CC2)C(=O)c2ccccc21
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[#7:7]1-[C:8]-[C:9]-[NH;D2;+0:10]-[C:11]-[C:12]-1>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[N;H0;D3;+0:10]1-[C:9]-[C:8]-[#7:7]-[C:12]-[C:11]-1)-[c:4](:[c:5]):[c:6]
null
[]
null
null
null
null
A 1.5 g portion of 3-chloro-2-piperazinyl-1,4-naphthoquinone and 1.26 g of 2-trifluoromethylbenzenesulfonyl chloride were reacted as described in Example 56, giving 1.53 g of the desired product, mp 122°-124° C. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Secondary amine.Sulfonyl halide
Tertiary amine
C1C[NH]CCN1
C1C[NH]CC[NH]1
C1C[NH]CC[NH]1.c1ccccc1.C1=CCc2ccccc2C1
HCl
null
null
null
O=C1C(Cl)=C(N2CCNCC2)C(=O)c2ccccc21.O=S(=O)(Cl)c1ccccc1C(F)(F)F>>O=C1C(Cl)=C(N2CCN(S(=O)(=O)c3ccccc3C(F)(F)F)CC2)C(=O)c2ccccc21
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-56336ee2ad824b1f9857b1d476eadee3
CC(=O)N(C(C)=O)C1=C(Cl)C(=O)c2ccccc2C1=O.Fc1ccc(N2CCNCC2)cc1>>CC(=O)N(C(C)=O)C1=C(N2CCN(c3ccc(F)cc3)CC2)C(=O)c2ccccc2C1=O
C(C)(=O)N(C(C)=O)C=1C(C2=CC=CC=C2C(C1Cl)=O)=O.FC1=CC=C(C=C1)N1CCNCC1>>C(C)(=O)N(C(C)=O)C=1C(C2=CC=CC=C2C(C1N1CCN(CC1)C1=CC=C(C=C1)F)=O)=O
Cl[C:9]1=[C:8]([N:4]([C:2]([CH3:1])=[O:3])[C:5]([CH3:6])=[O:7])[C:31](=[O:32])[c:30]2[c:25]([cH:26][cH:27][cH:28][cH:29]2)[C:23]1=[O:24].[NH:10]1[CH2:11][CH2:12][N:13]([c:14]2[cH:15][cH:16][c:17]([F:18])[cH:19][cH:20]2)[CH2:21][CH2:22]1>>[CH3:1][C:2](=[O:3])[N:4]([C:5]([CH3:6])=[O:7])[C:8]1=[C:9]([N:10]2[CH2:11][CH2:12...
CC(=O)N(C(C)=O)C1=C(Cl)C(=O)c2ccccc2C1=O.Fc1ccc(N2CCNCC2)cc1
CC(=O)N(C(C)=O)C1=C(N2CCN(c3ccc(F)cc3)CC2)C(=O)c2ccccc2C1=O
null
null
C(C)O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
d4a0d8c63c5bbf8e6b2a19dd3b1761c1fda17365ba7c27585f8e97bb31c6dca1
2f1af1bc2b6a104816ee6e304bb76145e9e36ef858bc716179b7b9df9c8858ef
O=C1C=C(N2CCN(c3ccccc3)CC2)C(=O)c2ccccc21
Cl-[C;H0;D3;+0:1]1=[C:2](-[#7:3](-[C:4](-[C;D1;H3:5])=[O;D1;H0:6])-[C:7](-[C;D1;H3:8])=[O;D1;H0:9])-[C:10](=[O;D1;H0:11])-[c:12]:[c:13]-[C:14]-1=[O;D1;H0:15].[#7:16]1-[C:17]-[C:18]-[NH;D2;+0:19]-[C:20]-[C:21]-1>>[C;D1;H3:5]-[C:4](=[O;D1;H0:6])-[#7:3](-[C:7](-[C;D1;H3:8])=[O;D1;H0:9])-[C:2]1=[C;H0;D3;+0:1](-[N;H0;D3;+0:...
null
[]
null
null
null
null
A mixture of 1.66 g of 2-[N,N-diacetylamino]-3-chloro-1,4-naphthoquinone and 1.441 g of 1-(4-fluorophenyl)piperazine in 50 ml of ethanol was refluxed overnight, then evaporated in vacuo. The residue was dissolved in dichloromethane, filtered through silica gel and eluted with chloroform:methanol (100:2). The eluent was...
10.6084/m9.figshare.5104873.v1
null
Enamine.Alkenyl halide.Ketone.Secondary amine
Enamine.Enamine
C1=CCc2ccccc2C1.C1CNCC[NH]1
C1C[NH]CC[NH]1.C1=CCc2ccccc2C1
C1C[NH]CC[NH]1.c1ccccc1.C1=CCc2ccccc2C1
HCl
C(C)O
null
null
CC(=O)N(C(C)=O)C1=C(Cl)C(=O)c2ccccc2C1=O.Fc1ccc(N2CCNCC2)cc1>C(C)O>CC(=O)N(C(C)=O)C1=C(N2CCN(c3ccc(F)cc3)CC2)C(=O)c2ccccc2C1=O
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-ce5069d4005549b6a217e8c95207166c
FC(F)(F)c1cccc(N2CCNCC2)c1.O=C1c2ccccc2C(=O)C2OC12>>O=C1C(O)=C(N2CCN(c3cccc(C(F)(F)F)c3)CC2)C(=O)c2ccccc21
O1C2C(C3=CC=CC=C3C(C21)=O)=O.FC(C=1C=C(C=CC1)N1CCNCC1)(F)F>>OC=1C(C2=CC=CC=C2C(C1N1CCN(CC1)C1=CC(=CC=C1)C(F)(F)F)=O)=O
[NH:6]1[CH2:7][CH2:8][N:9]([c:10]2[cH:11][cH:12][cH:13][c:14]([C:15]([F:16])([F:17])[F:18])[cH:19]2)[CH2:20][CH2:21]1.[O:1]=[C:2]1[CH:3]2[O:4][CH:5]2[C:22](=[O:23])[c:24]2[cH:25][cH:26][cH:27][cH:28][c:29]21>>[O:1]=[C:2]1[C:3]([OH:4])=[C:5]([N:6]2[CH2:7][CH2:8][N:9]([c:10]3[cH:11][cH:12][cH:13][c:14]([C:15]([F:16])([F:...
FC(F)(F)c1cccc(N2CCNCC2)c1.O=C1c2ccccc2C(=O)C2OC12
O=C1C(O)=C(N2CCN(c3cccc(C(F)(F)F)c3)CC2)C(=O)c2ccccc21
null
null
C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
d159dfad41809e764977fe62b321d77c82e03faa2312b9af50da554c86691eac
9eb32644625dfa7918a42cd35d30ff1a368832023364da9d9ecebca843a55107
O=C1C=C(N2CCN(c3ccccc3)CC2)C(=O)c2ccccc21
[#7:1]1-[C:2]-[C:3]-[NH;D2;+0:4]-[C:5]-[C:6]-1.[O;D1;H0:7]=[C:8]1-[c:9]:[c:10]-[C:11](=[O;D1;H0:12])-[CH;D3;+0:13]2-[O;H0;D2;+0:14]-[CH;D3;+0:15]-1-2>>[O;D1;H0:7]=[C:8]1-[c:9]:[c:10]-[C:11](=[O;D1;H0:12])-[C;H0;D3;+0:13](-[N;H0;D3;+0:4]2-[C:3]-[C:2]-[#7:1]-[C:6]-[C:5]-2)=[C;H0;D3;+0:15]-1-[OH;D1;+0:14]
29.9
[{"value": 29.9, "product": "OC=1C(C2=CC=CC=C2C(C1N1CCN(CC1)C1=CC(=CC=C1)C(F)(F)F)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
20
HOUR
A mixture of 1.74 g of 2,3-epoxy-2,3-dihydro-1,4-naphthoquinone and 2.30 g of N-[3-(trifluoromethyl)phenyl]piperazine in 100 ml of absolute ethanol was stirred for 20 hours, then evaporated. The residue was dissolved in dichloromethane, filtered through hydrous magnesium silicate and then chromatographed on silica gel,...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ketone.Ether.Secondary amine
Enamine.Ketone.Ketone.Enol
C1CNCC[NH]1.c1ccc2c(c1)CC1OC1C2
C1C[NH]CC[NH]1.C1=CCc2ccccc2C1
C1C[NH]CC[NH]1.c1ccccc1.C1=CCc2ccccc2C1
null
C(C)O
null
20
FC(F)(F)c1cccc(N2CCNCC2)c1.O=C1c2ccccc2C(=O)C2OC12>C(C)O>O=C1C(O)=C(N2CCN(c3cccc(C(F)(F)F)c3)CC2)C(=O)c2ccccc21
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-dbaeee1d10774d5b9ecd93a63368c816
CNCCN(C)Cc1ccccc1.O=C1c2ccccc2C(=O)C2OC12>>CN(CCN(C)C1=C(O)C(=O)c2ccccc2C1=O)Cc1ccccc1
O1C2C(C3=CC=CC=C3C(C21)=O)=O.C(C1=CC=CC=C1)N(CCNC)C>>OC=1C(C2=CC=CC=C2C(C1N(CCN(CC1=CC=CC=C1)C)C)=O)=O
[CH3:1][N:2]([CH2:3][CH2:4][NH:5][CH3:6])[CH2:20][c:21]1[cH:22][cH:23][cH:24][cH:25][cH:26]1.[CH:7]12[CH:8]([O:9]1)[C:10](=[O:11])[c:12]1[cH:13][cH:14][cH:15][cH:16][c:17]1[C:18]2=[O:19]>>[CH3:1][N:2]([CH2:3][CH2:4][N:5]([CH3:6])[C:7]1=[C:8]([OH:9])[C:10](=[O:11])[c:12]2[cH:13][cH:14][cH:15][cH:16][c:17]2[C:18]1=[O:19]...
CNCCN(C)Cc1ccccc1.O=C1c2ccccc2C(=O)C2OC12
CN(CCN(C)C1=C(O)C(=O)c2ccccc2C1=O)Cc1ccccc1
null
null
C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
0028c448e315ec41f72d3c8a14ffdb1089cc2267edd908074c6e06b32c404332
9eb32644625dfa7918a42cd35d30ff1a368832023364da9d9ecebca843a55107
O=C1C=C(NCCNCc2ccccc2)C(=O)c2ccccc21
[C:1]-[C:2]-[NH;D2;+0:3]-[C;D1;H3:4].[O;D1;H0:5]=[C:6]1-[c:7]:[c:8]-[C:9](=[O;D1;H0:10])-[CH;D3;+0:11]2-[O;H0;D2;+0:12]-[CH;D3;+0:13]-1-2>>[C:1]-[C:2]-[N;H0;D3;+0:3](-[C;D1;H3:4])-[C;H0;D3;+0:11]1=[C;H0;D3;+0:13](-[OH;D1;+0:12])-[C:6](=[O;D1;H0:5])-[c:7]:[c:8]-[C:9]-1=[O;D1;H0:10]
null
[]
null
null
20
HOUR
A mixture of 2.61 g of 2,3-epoxy-2,3-dihydro-1,4-naphthoquinone, 2.67 g of N-benzyl-N,N'-dimethylethylenediamine and 150 ml of absolute ethanol was stirred for 20 hours, then concentrated to one-half its original volume and refrigerated overnight. The solvent was removed, the residue dissolved in dichloromethane and pa...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ketone.Ether.Secondary amine
Enamine.Ketone.Ketone.Enol
c1ccc2c(c1)CC1OC1C2
C1=CCc2ccccc2C1
C1=CCc2ccccc2C1.c1ccccc1
null
C(C)O
null
20
CNCCN(C)Cc1ccccc1.O=C1c2ccccc2C(=O)C2OC12>C(C)O>CN(CCN(C)C1=C(O)C(=O)c2ccccc2C1=O)Cc1ccccc1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-76e2664d978c4a2197ffbdd9fcee90d3
O=C1c2ccccc2C(=O)C2OC12.O=CN1CCNCC1>>O=CN1CCN(C2=C(O)C(=O)c3ccccc3C2=O)CC1
O1C2C(C3=CC=CC=C3C(C21)=O)=O.N1(CCNCC1)C=O>>OC1=C(C(C2=CC=CC=C2C1=O)=O)N1CCN(CC1)C=O
[CH:7]12[CH:8]([O:9]1)[C:10](=[O:11])[c:12]1[cH:13][cH:14][cH:15][cH:16][c:17]1[C:18]2=[O:19].[O:1]=[CH:2][N:3]1[CH2:4][CH2:5][NH:6][CH2:20][CH2:21]1>>[O:1]=[CH:2][N:3]1[CH2:4][CH2:5][N:6]([C:7]2=[C:8]([OH:9])[C:10](=[O:11])[c:12]3[cH:13][cH:14][cH:15][cH:16][c:17]3[C:18]2=[O:19])[CH2:20][CH2:21]1
O=C1c2ccccc2C(=O)C2OC12.O=CN1CCNCC1
O=CN1CCN(C2=C(O)C(=O)c3ccccc3C2=O)CC1
null
null
C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
3d62cca493370f2e39512df12599eb3940fa8a217b80897143eb7507fe49beac
9eb32644625dfa7918a42cd35d30ff1a368832023364da9d9ecebca843a55107
O=C1C=C(N2CCNCC2)C(=O)c2ccccc21
[#7:1]1-[C:2]-[C:3]-[NH;D2;+0:4]-[C:5]-[C:6]-1.[O;D1;H0:7]=[C:8]1-[c:9]:[c:10]-[C:11](=[O;D1;H0:12])-[CH;D3;+0:13]2-[O;H0;D2;+0:14]-[CH;D3;+0:15]-1-2>>[O;D1;H0:7]=[C:8]1-[c:9]:[c:10]-[C:11](=[O;D1;H0:12])-[C;H0;D3;+0:13](-[N;H0;D3;+0:4]2-[C:3]-[C:2]-[#7:1]-[C:6]-[C:5]-2)=[C;H0;D3;+0:15]-1-[OH;D1;+0:14]
null
[]
null
null
20
HOUR
A mixture of 3.48 g of 2,3-epoxy-2,3-dihydro-1,4-naphthoquinone, 2.28 of 1-piperazinecarboxaldehyde and 200 ml of absolute ethanol was stirred for 20 hours, then concentrated to one-half its original volume and refrigerated overnight. The solid was collected and recrystallized from dichloromethane/ethanol, giving 2.65 ...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ketone.Ether.Secondary amine
Enamine.Ketone.Ketone.Enol
c1ccc2c(c1)CC1OC1C2.C1C[NH]CCN1
C1C[NH]CC[NH]1.C1=CCc2ccccc2C1
C1C[NH]CC[NH]1.C1=CCc2ccccc2C1
null
C(C)O
null
20
O=C1c2ccccc2C(=O)C2OC12.O=CN1CCNCC1>C(C)O>O=CN1CCN(C2=C(O)C(=O)c3ccccc3C2=O)CC1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-4a85381d106d486ab137598d3b983c45
O=C1c2ccccc2C(=O)C2OC12.c1ccc2oc(N3CCNCC3)nc2c1>>O=C1C(O)=C(N2CCN(c3nc4ccccc4o3)CC2)C(=O)c2ccccc21
O1C2C(C3=CC=CC=C3C(C21)=O)=O.N1(CCNCC1)C=1OC2=C(N1)C=CC=C2>>O1C(=NC2=C1C=CC=C2)N2CCN(CC2)C=2C(C1=CC=CC=C1C(C2O)=O)=O
[O:1]=[C:2]1[CH:3]2[O:4][CH:5]2[C:21](=[O:22])[c:23]2[cH:24][cH:25][cH:26][cH:27][c:28]21.[NH:6]1[CH2:7][CH2:8][N:9]([c:10]2[n:11][c:12]3[cH:13][cH:14][cH:15][cH:16][c:17]3[o:18]2)[CH2:19][CH2:20]1>>[O:1]=[C:2]1[C:3]([OH:4])=[C:5]([N:6]2[CH2:7][CH2:8][N:9]([c:10]3[n:11][c:12]4[cH:13][cH:14][cH:15][cH:16][c:17]4[o:18]3)...
O=C1c2ccccc2C(=O)C2OC12.c1ccc2oc(N3CCNCC3)nc2c1
O=C1C(O)=C(N2CCN(c3nc4ccccc4o3)CC2)C(=O)c2ccccc21
null
null
C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
d159dfad41809e764977fe62b321d77c82e03faa2312b9af50da554c86691eac
9eb32644625dfa7918a42cd35d30ff1a368832023364da9d9ecebca843a55107
O=C1C=C(N2CCN(c3nc4ccccc4o3)CC2)C(=O)c2ccccc21
[#7:1]1-[C:2]-[C:3]-[NH;D2;+0:4]-[C:5]-[C:6]-1.[O;D1;H0:7]=[C:8]1-[c:9]:[c:10]-[C:11](=[O;D1;H0:12])-[CH;D3;+0:13]2-[O;H0;D2;+0:14]-[CH;D3;+0:15]-1-2>>[O;D1;H0:7]=[C:8]1-[c:9]:[c:10]-[C:11](=[O;D1;H0:12])-[C;H0;D3;+0:13](-[N;H0;D3;+0:4]2-[C:3]-[C:2]-[#7:1]-[C:6]-[C:5]-2)=[C;H0;D3;+0:15]-1-[OH;D1;+0:14]
14.2
[{"value": 14.2, "product": "O1C(=NC2=C1C=CC=C2)N2CCN(CC2)C=2C(C1=CC=CC=C1C(C2O)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
18
HOUR
A mixture of 3.48 g of 2,3-epoxy-2,3-dihydro-1,4-naphthoquinone, 2.03 g of 2-(1-piperazinyl)benzoxazole and 200 ml of absolute ethanol was stirred for 18 hours and then filtered. The filtrate was concentrated to dryness and the residue flash chromatographed, eluting with dichloromethane, then 1% methanol in dichloromet...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ketone.Ether.Secondary amine
Enamine.Ketone.Ketone.Enol
c1ccc2c(c1)CC1OC1C2.C1CNCC[NH]1
C1C[NH]CC[NH]1.C1=CCc2ccccc2C1
C1C[NH]CC[NH]1.c1ccc2ocnc2c1.C1=CCc2ccccc2C1
null
C(C)O
null
18
O=C1c2ccccc2C(=O)C2OC12.c1ccc2oc(N3CCNCC3)nc2c1>C(C)O>O=C1C(O)=C(N2CCN(c3nc4ccccc4o3)CC2)C(=O)c2ccccc21
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-befc1a5140b3477ba8bc5c430cf45d86
CCOC(=O)N1CCNCC1.O=C1c2ccccc2C(=O)C2OC12>>CCOC(=O)N1CCN(C2=C(O)C(=O)c3ccccc3C2=O)CC1
O1C2C(C3=CC=CC=C3C(C21)=O)=O.CCOC(=O)N1CCNCC1>>OC1=C(C(C2=CC=CC=C2C1=O)=O)N1CCN(CC1)C(=O)OCC
[CH3:1][CH2:2][O:3][C:4](=[O:5])[N:6]1[CH2:7][CH2:8][NH:9][CH2:23][CH2:24]1.[CH:10]12[CH:11]([O:12]1)[C:13](=[O:14])[c:15]1[cH:16][cH:17][cH:18][cH:19][c:20]1[C:21]2=[O:22]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[N:6]1[CH2:7][CH2:8][N:9]([C:10]2=[C:11]([OH:12])[C:13](=[O:14])[c:15]3[cH:16][cH:17][cH:18][cH:19][c:20]3[C:21]2=...
CCOC(=O)N1CCNCC1.O=C1c2ccccc2C(=O)C2OC12
CCOC(=O)N1CCN(C2=C(O)C(=O)c3ccccc3C2=O)CC1
null
null
C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
3d62cca493370f2e39512df12599eb3940fa8a217b80897143eb7507fe49beac
9eb32644625dfa7918a42cd35d30ff1a368832023364da9d9ecebca843a55107
O=C1C=C(N2CCNCC2)C(=O)c2ccccc21
[#7:1]1-[C:2]-[C:3]-[NH;D2;+0:4]-[C:5]-[C:6]-1.[O;D1;H0:7]=[C:8]1-[c:9]:[c:10]-[C:11](=[O;D1;H0:12])-[CH;D3;+0:13]2-[O;H0;D2;+0:14]-[CH;D3;+0:15]-1-2>>[O;D1;H0:7]=[C:8]1-[c:9]:[c:10]-[C:11](=[O;D1;H0:12])-[C;H0;D3;+0:13](-[N;H0;D3;+0:4]2-[C:3]-[C:2]-[#7:1]-[C:6]-[C:5]-2)=[C;H0;D3;+0:15]-1-[OH;D1;+0:14]
44.9
[{"value": 44.9, "product": "OC1=C(C(C2=CC=CC=C2C1=O)=O)N1CCN(CC1)C(=O)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
24
HOUR
A mixture of 1.174 g of 2,3-epoxy-2,3-dihydro-1,4-naphthoquinone, 1.58 g of ethyl-N-piperazinocarboxylate and 100 ml of absolute ethanol was stirred for 24 hours, then evaporated. The residue was chromatographed on silica gel, eluting with 5% methanol in chloroform, giving 1.0 g of the desired product, mp 115°-118° C. ...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ketone.Ether.Secondary amine
Enamine.Ketone.Ketone.Enol
C1C[NH]CCN1.c1ccc2c(c1)CC1OC1C2
C1C[NH]CC[NH]1.C1=CCc2ccccc2C1
C1C[NH]CC[NH]1.C1=CCc2ccccc2C1
null
C(C)O
null
24
CCOC(=O)N1CCNCC1.O=C1c2ccccc2C(=O)C2OC12>C(C)O>CCOC(=O)N1CCN(C2=C(O)C(=O)c3ccccc3C2=O)CC1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-40f86100453649baaaad16821658abaf
CC(=O)c1ccc(Cl)nc1.[N-]=[N+]=[N-]>>CC(=O)c1ccc2nnnn2c1
Cl.ClC1=NC=C(C=C1)C(C)=O.[N-]=[N+]=[N-].[Na+].C(C)O>>C(C)(=O)C=1C=CC=2N(C1)N=NN2
Cl[c:7]1[cH:6][cH:5][c:4]([C:2]([CH3:1])=[O:3])[cH:12][n:11]1.[N-:8]=[N+:10]=[N-:9]>>[CH3:1][C:2](=[O:3])[c:4]1[cH:5][cH:6][c:7]2[n:8][n:9][n:10][n:11]2[cH:12]1
CC(=O)c1ccc(Cl)nc1.[N-]=[N+]=[N-]
CC(=O)c1ccc2nnnn2c1
null
null
O
Aromatic Heterocycle Formation
OtherReaction
60967d0a10df13474ce7ef580cb6a95c4a598735845b09f5aad8d662786255e3
155f764f095c8454a4ad08aaa42f1abcb15d5bc1d4f122e4bcc624dd834362f2
c1ccn2nnnc2c1
Cl-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](-[C:5](-[C;D1;H3:6])=[O;D1;H0:7]):[c:8]:[n;H0;D2;+0:9]:1.[N-;H0;D1:10]=[N+;H0;D2:11]=[N-;H0;D1:12]>>[C;D1;H3:6]-[C:5](=[O;D1;H0:7])-[c:4]1:[c:8]:[n;H0;D3;+0:9]2:[n;H0;D2;+0:11]:[n;H0;D2;+0:12]:[n;H0;D2;+0:10]:[c;H0;D3;+0:1]:2:[c:2]:[c:3]:1
null
[]
null
null
null
null
To a stirred solution of 8.4 gm. (51.6 mmoles) of 2-chloro-5-acetylpyridine and 8.4 gm. (129 mmoles) of sodium azide in 150 ml. of ethanol and 150 ml. of water was added 75 ml. of 10% HCl over a period of 20min. The reaction mixture was then heated to reflux for 18 hours, cooled in an ice bath and the resulting crystal...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1ccncc1
c1ccn2nnnc2c1
c1ccn2nnnc2c1
Other
O
null
null
CC(=O)c1ccc(Cl)nc1.[N-]=[N+]=[N-]>O>CC(=O)c1ccc2nnnn2c1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-8ec6bc0ba583456dba19b4ce1259fcc1
O=C(O)c1ccc(F)nc1>>CC(=O)c1ccc(F)nc1
FC1=NC=C(C=C1)C(=O)O.C[Li]>>C(C)(=O)C=1C=CC(=NC1)F
O[C:2](=[O:3])[c:4]1[cH:5][cH:6][c:7]([F:8])[n:9][cH:10]1>>[CH3:1][C:2](=[O:3])[c:4]1[cH:5][cH:6][c:7]([F:8])[n:9][cH:10]1
O=C(O)c1ccc(F)nc1
CC(=O)c1ccc(F)nc1
null
null
CCOCC
Functional Group Interconversion
OtherReaction
e9c3cedbcda67d0df54f9106bb41f00b64c34f45c22680bd429b0c3cd51664a5
6a71bb5a71b59feeb4f6a39b1b66fa450a058b64b0a3909e1a51c22473a141c5
c1ccncc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]:[#7;a:6]:[c:7]>>[C;D1;H3:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]:[#7;a:6]:[c:7]
null
[]
null
null
2
HOUR
To suspension of 20 gm. (]42 mmoles) of 2-fluoro-5-pyridinecarboxylic acid (J.Am. Chem. Soc., 71, 1125 (1949)) in 750 ml. of ether, stirred and cooled in ice, was added 225 ml. of 1.6 M methyl lithium (360 mmoles) in ether over 1 hr. The reaction was stirred for an additional 2 hr., then 300 ml. of ice water was added....
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Ketone
null
null
c1ccncc1
null
CCOCC
null
2
O=C(O)c1ccc(F)nc1>CCOCC>CC(=O)c1ccc(F)nc1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-b71060c88f1e48328aff893e3244c153
N#CCc1coc2ccccc12>>NCCc1coc2ccccc12
C(#N)CC=1C2=C(OC1)C=CC=C2.[H-].[Al+3].[Li+].[H-].[H-].[H-].O>>O1C2=C(C(=C1)CCN)C=CC=C2
[N:1]#[C:2][CH2:3][c:4]1[cH:5][o:6][c:7]2[cH:8][cH:9][cH:10][cH:11][c:12]12>>[NH2:1][CH2:2][CH2:3][c:4]1[cH:5][o:6][c:7]2[cH:8][cH:9][cH:10][cH:11][c:12]12
N#CCc1coc2ccccc12
NCCc1coc2ccccc12
null
null
CCOCC.C(C)OCC
Reduction
Reduction of nitrile to amine
65bec2d9f430701d30dc9fcbe1c5418f3dfa174d67be035c50edfc71895dc9c7
e8d1bc928b94bd4f5bf4b23363ce8f88b1ce7d146ba93829e7b8ad8dbe0007a7
c1ccc2occc2c1
[#8;a:1]:[c:2]:[c:3]-[C:4]-[C;H0;D2;+0:5]#[N;H0;D1;+0:6]>>[#8;a:1]:[c:2]:[c:3]-[C:4]-[CH2;D2;+0:5]-[NH2;D1;+0:6]
79.4
[{"value": 79.4, "product": "O1C2=C(C(=C1)CCN)C=CC=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 3.97 g (0.025 mole) of 3-cyanomethylbenzo[b]furan in 200 mL of diethyl ether was slowly added to a refluxing suspension of 3.84 g (0.1 mole) of lithium aluminum hydride in 400 mL of ether. The reaction was heated 3 hrs., cooled and water was slowly added. The suspension was filtered through a pad of filte...
10.6084/m9.figshare.5104873.v1
null
Nitrile
Primary amine
null
null
c1ccc2occc2c1
null
CCOCC.C(C)OCC
null
null
N#CCc1coc2ccccc12>CCOCC.C(C)OCC>NCCc1coc2ccccc12
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-9b18f248c70e4a0392e77af9b435df2f
CCOC=O.NCCc1coc2ccccc12>>O=CNCCc1coc2ccccc12
O1C2=C(C(=C1)CCN)C=CC=C2.C(=O)OCC.Cl>>C(=O)NCCC=1C2=C(OC1)C=CC=C2
CCO[CH:2]=[O:1].[NH2:3][CH2:4][CH2:5][c:6]1[cH:7][o:8][c:9]2[cH:10][cH:11][cH:12][cH:13][c:14]12>>[O:1]=[CH:2][NH:3][CH2:4][CH2:5][c:6]1[cH:7][o:8][c:9]2[cH:10][cH:11][cH:12][cH:13][c:14]12
CCOC=O.NCCc1coc2ccccc12
O=CNCCc1coc2ccccc12
null
null
null
Acylation
OtherReaction
003d6e284475e7d4fe43f9e91e4ad7ca9bf4d7f2029a8fe4e8eed7dbde0fdef0
25423bd5162c5be916302ae1ac632b1f2d5d912d0ee7eadf1b5b1259507dc6c3
c1ccc2occc2c1
C-C-O-[CH;D2;+0:1]=[O;D1;H0:2].[C:3]-[C:4]-[NH2;D1;+0:5]>>[C:3]-[C:4]-[NH;D2;+0:5]-[CH;D2;+0:1]=[O;D1;H0:2]
null
[]
null
null
null
null
A solution of 2.35 g (0.015 mole) of 2-(3-benzo[b]furanyl)ethylamine and 5 mL of ethyl formate was heated at 60° C. for 3 hours, poured into 2N HCl and washed with methylene chloride which in turn was washed with 5% sodium hydroxide (w/v), dried (MgSO4), filtered and concentrated to give 2.70 g of product. Conditions: ...
10.6084/m9.figshare.5104873.v1
null
Ether.Primary amine
Secondary amide
null
null
c1ccc2occc2c1
HO-
null
null
null
CCOC=O.NCCc1coc2ccccc12>>O=CNCCc1coc2ccccc12
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-d376c969a22a4ad9a4185fd147ab4198
CC(=O)Cl.O=Cc1ccc(CO)cc1>>CC(=O)OCc1ccc(C=O)cc1
OCC1=CC=C(C=O)C=C1.C(C)N(CC)CC.C(C)(=O)Cl>>C(C)(=O)OCC1=CC=C(C=O)C=C1
Cl[C:2]([CH3:1])=[O:3].[OH:4][CH2:5][c:6]1[cH:7][cH:8][c:9]([CH:10]=[O:11])[cH:12][cH:13]1>>[CH3:1][C:2](=[O:3])[O:4][CH2:5][c:6]1[cH:7][cH:8][c:9]([CH:10]=[O:11])[cH:12][cH:13]1
CC(=O)Cl.O=Cc1ccc(CO)cc1
CC(=O)OCc1ccc(C=O)cc1
null
null
ClCCl
Acylation
Schotten-Baumann to ester
6cefe709828c5bd4655f254e75d5dff9e8876e192e7dd47256c1bc0067bc5291
d8a7643b81ed07a6f633aa99465180dfa0565e61ae25aef36338ebb9837c9cef
c1ccccc1
Cl-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[OH;D1;+0:4]-[C:5]-[c:6]>>[C;D1;H3:2]-[C;H0;D3;+0:1](=[O;D1;H0:3])-[O;H0;D2;+0:4]-[C:5]-[c:6]
67.6
[{"value": 67.6, "product": "C(C)(=O)OCC1=CC=C(C=O)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
54.2 g of 4-hydroxymethylbenzaldehyde, together with 40 g of triethylamine, are dissolved in 350 ml of dichloromethane. After the dropwise addition of 31.2 g of acetyl chloride at 0° to 5° C., the reaction mixture is allowed to stand overnight at room temperature. Thereafter, the precipitated triethylammonium chloride ...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary alcohol
Ester
null
null
c1ccccc1
HCl
ClCCl
null
8
CC(=O)Cl.O=Cc1ccc(CO)cc1>ClCCl>CC(=O)OCc1ccc(C=O)cc1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-4262ef1b8922496ebfefb960ef4290bd
CC(=O)CCl.Nc1nccc2c(Cl)cccc12>>Cc1cn2ccc3c(Cl)cccc3c2n1
ClC1=C2C=CN=C(C2=CC=C1)N.ClCC(C)=O.C([O-])(O)=O.[Na+]>>ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3)C
O=[C:2]([CH3:1])[CH2:3]Cl.[n:4]1[cH:5][cH:6][c:7]2[c:8]([Cl:9])[cH:10][cH:11][cH:12][c:13]2[c:14]1[NH2:15]>>[CH3:1][c:2]1[cH:3][n:4]2[cH:5][cH:6][c:7]3[c:8]([Cl:9])[cH:10][cH:11][cH:12][c:13]3[c:14]2[n:15]1
CC(=O)CCl.Nc1nccc2c(Cl)cccc12
Cc1cn2ccc3c(Cl)cccc3c2n1
null
null
C(C)O
Aromatic Heterocycle Formation
OtherReaction
78935ce312554100564931917e18f278a2f0536f5f6cc66905362a94d2708db3
9e77d52183fdbe84f0d2ab96039aaf521caea9340e743bdc6436175f1a3bbdb6
c1ccc2c(c1)ccn1ccnc21
Cl-[CH2;D2;+0:1]-[C;H0;D3;+0:2](=O)-[C;D1;H3:3].[NH2;D1;+0:4]-[c:5](:[c:6]):[n;H0;D2;+0:7]:[c:8]:[c:9]>>[C;D1;H3:3]-[c;H0;D3;+0:2]1:[cH;D2;+0:1]:[n;H0;D3;+0:7](:[c:8]:[c:9]):[c:5](:[c:6]):[n;H0;D2;+0:4]:1
82.4
[{"value": 82.4, "product": "ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
null
null
A mixture of 5-chloro-1-aminoisoquinoline (2.8 g), chloroacetone (5.4 g) and sodium bicarbonate (7.6 g) in anhydrous ethanol (35 ml) was heated at 60° C. for 16 hours and filtered by suction. The filtrate was evaporated in vacuo and the residual solid was washed with ethanol to give 7-chloro-2-methylimidazo[2,1-a]isoqu...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ketone.Primary amine
null
c1ccc2cnccc2c1
c1ccc2c(c1)ccn1ccnc21
c1ccc2c(c1)ccn1ccnc21
HCl
C(C)O
60
null
CC(=O)CCl.Nc1nccc2c(Cl)cccc12>C(C)O>Cc1cn2ccc3c(Cl)cccc3c2n1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-181a7e40fb93472d9d081e58c92d33b5
C=O.CNC.Cc1cn2ccc3c(Cl)cccc3c2n1>>Cc1nc2c3cccc(Cl)c3ccn2c1CN(C)C
[OH-].[Na+].C=O.CNC.ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3)C>>ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3CN(C)C)C
O=[CH2:19].[CH3:16][NH:17][CH3:18].[CH3:1][c:2]1[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][c:9]([Cl:10])[c:11]3[cH:12][cH:13][n:14]2[cH:15]1>>[CH3:1][c:2]1[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][c:9]([Cl:10])[c:11]3[cH:12][cH:13][n:14]2[c:15]1[CH2:16][N:17]([CH3:18])[CH3:19]
C=O.CNC.Cc1cn2ccc3c(Cl)cccc3c2n1
Cc1nc2c3cccc(Cl)c3ccn2c1CN(C)C
null
null
C(C)(=O)O
Heteroatom Alkylation and Arylation
OtherReaction
f926e897ee7bad83fc9082ae29360b37528a72be55856903bdf8153b0d2166fe
e1fdef8fde1c506d7c9deb8fd5e6f322eceea2abce3167abcf412a1fa4fd5443
c1ccc2c(c1)ccn1ccnc21
O=[CH2;D1;+0:1].[C;D1;H3:2]-[NH;D2;+0:3]-[CH3;D1;+0:4].[C;D1;H3:5]-[c:6]1:[#7;a:7]:[c:8](:[c:9]):[#7;a:10](:[c:11]):[cH;D2;+0:12]:1>>[C;D1;H3:2]-[N;H0;D3;+0:3](-[CH3;D1;+0:1])-[CH2;D2;+0:4]-[c;H0;D3;+0:12]1:[#7;a:10](:[c:11]):[c:8](:[c:9]):[#7;a:7]:[c:6]:1-[C;D1;H3:5]
71.2
[{"value": 71.2, "product": "ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3CN(C)C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
50
CELSIUS
3.5
HOUR
To a solution of 37% aqueous formaldehyde (0.42 g) and 50% aqueous dimethylamine (0.46 g) in acetic acid (3.2 ml) was added 7-chloro-2-methylimidazo[2,1-a]isoquinoline (1 g) and the mixture was warmed at 50° C. with stirring for 3.5 hours. The solution was poured into ice water and neutralized with an aqueous solution ...
10.6084/m9.figshare.5104873.v1
null
Formaldehyde.Secondary amine
Tertiary amine
c1ccc2c(c1)ccn1ccnc21
c1ccc2c(c1)ccn1ccnc21
c1ccc2c(c1)ccn1ccnc21
HO-
C(C)(=O)O
50
3.5
C=O.CNC.Cc1cn2ccc3c(Cl)cccc3c2n1>C(C)(=O)O>Cc1nc2c3cccc(Cl)c3ccn2c1CN(C)C
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-05a503c69e62474e8c0cab369e6ea2f1
COS(=O)(=O)OC.Cc1nc2c3ccccc3ccn2c1CN(C)C>>COS(=O)(=O)[O-].Cc1nc2c3ccccc3ccn2c1C[N+](C)(C)C
CN(C)CC1=C(N=C2N1C=CC1=CC=CC=C21)C.S(=O)(=O)(OC)OC.C(C)OCC>>COS(=O)(=O)[O-].CC=1N=C2N(C=CC3=CC=CC=C23)C1C[N+](C)(C)C
[CH3:1][O:2][S:3](=[O:4])(=[O:5])[O:6][CH3:23].[CH3:7][c:8]1[n:9][c:10]2[c:11]3[cH:12][cH:13][cH:14][cH:15][c:16]3[cH:17][cH:18][n:19]2[c:20]1[CH2:21][N:22]([CH3:24])[CH3:25]>>[CH3:1][O:2][S:3](=[O:4])(=[O:5])[O-:6].[CH3:7][c:8]1[n:9][c:10]2[c:11]3[cH:12][cH:13][cH:14][cH:15][c:16]3[cH:17][cH:18][n:19]2[c:20]1[CH2:21][...
COS(=O)(=O)OC.Cc1nc2c3ccccc3ccn2c1CN(C)C
COS(=O)(=O)[O-].Cc1nc2c3ccccc3ccn2c1C[N+](C)(C)C
null
null
O1CCCC1
Functional Group Interconversion
OtherReaction
c1c361ee4cbadaf5c6784ce94893dc199b85d8bd1f54519979f4b44d8dfd8b3e
5a8d30abc7481f1c446ec3891ae2e6d38df9cf7a08165b843f1d24fc50c4b9cd
c1ccc2c(c1)ccn1ccnc21
[#7;a:1]:[c:2](-[C:3]-[N;H0;D3;+0:4](-[C;D1;H3:5])-[C;D1;H3:6]):[c:7]:[#7;a:8].[C;D1;H3:9]-[#8:10]-[#16:11](=[O;D1;H0:12])(=[O;D1;H0:13])-[O;H0;D2;+0:14]-[CH3;D1;+0:15]>>[#7;a:1]:[c:2](-[C:3]-[N+;H0;D4:4](-[C;D1;H3:5])(-[C;D1;H3:6])-[CH3;D1;+0:15]):[c:7]:[#7;a:8].[C;D1;H3:9]-[#8:10]-[#16:11](-[O-;H0;D1:14])(=[O;D1;H0:1...
null
[]
null
null
null
null
A solution of 3-dimethylaminomethyl-2-methylimidazo[2,1-a]isoquinoline (7.7 g) in tetrahydrofuran (20 ml) was added dropwise to a solution of dimethyl sulfate (15 ml) in tetrahydrofuran (40 ml) with ice-cooling and stirring, and the mixture was stirred for 2 hours under the same conditions. To the reaction mixture was ...
10.6084/m9.figshare.5104873.v1
null
Tertiary amine
null
null
null
c1ccc2c(c1)ccn1ccnc21
null
O1CCCC1
null
null
COS(=O)(=O)OC.Cc1nc2c3ccccc3ccn2c1CN(C)C>O1CCCC1>COS(=O)(=O)[O-].Cc1nc2c3ccccc3ccn2c1C[N+](C)(C)C
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-93256b0b1b2d4e259b6a55c562dc49d1
CI.Cc1nc2c3ccc(Cl)cc3ccn2c1CN(C)C>>Cc1nc2c3ccc(Cl)cc3ccn2c1C[N+](C)(C)C.[I-]
CI.ClC=1C=C2C=CN3C(C2=CC1)=NC(=C3CN(C)C)C>>[I-].ClC=1C=C2C=CN3C(C2=CC1)=NC(=C3C[N+](C)(C)C)C
[CH3:18][I:21].[CH3:1][c:2]1[n:3][c:4]2[c:5]3[cH:6][cH:7][c:8]([Cl:9])[cH:10][c:11]3[cH:12][cH:13][n:14]2[c:15]1[CH2:16][N:17]([CH3:19])[CH3:20]>>[CH3:1][c:2]1[n:3][c:4]2[c:5]3[cH:6][cH:7][c:8]([Cl:9])[cH:10][c:11]3[cH:12][cH:13][n:14]2[c:15]1[CH2:16][N+:17]([CH3:18])([CH3:19])[CH3:20].[I-:21]
CI.Cc1nc2c3ccc(Cl)cc3ccn2c1CN(C)C
Cc1nc2c3ccc(Cl)cc3ccn2c1C[N+](C)(C)C.[I-]
null
null
C(C)O
Functional Group Interconversion
OtherReaction
c1c361ee4cbadaf5c6784ce94893dc199b85d8bd1f54519979f4b44d8dfd8b3e
5a8d30abc7481f1c446ec3891ae2e6d38df9cf7a08165b843f1d24fc50c4b9cd
c1ccc2c(c1)ccn1ccnc21
[#7;a:1]:[c:2](-[C:3]-[N;H0;D3;+0:4](-[C;D1;H3:5])-[C;D1;H3:6]):[c:7]:[#7;a:8].[CH3;D1;+0:9]-[I;H0;D1;+0:10]>>[#7;a:1]:[c:2](-[C:3]-[N+;H0;D4:4](-[C;D1;H3:5])(-[C;D1;H3:6])-[CH3;D1;+0:9]):[c:7]:[#7;a:8].[I-;H0;D0:10]
84.2
[{"value": 84.2, "product": "[I-].ClC=1C=C2C=CN3C(C2=CC1)=NC(=C3C[N+](C)(C)C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
14
HOUR
Methyliodide (1.7 g) was added dropwise to a solution of 8-chloro-3-dimethylaminomethyl-2-methylimidazo[2,1-a]isoquinoline (2.8 g) in ethanol (34 ml) at room temperature and the mixture was stirred for 14 hours. The resulting precipitate was collected by filtration, washed with ethanol and dried in a desiccator to give...
10.6084/m9.figshare.5104873.v1
null
Tertiary amine
null
null
null
c1ccc2c(c1)ccn1ccnc21
null
C(C)O
null
14
CI.Cc1nc2c3ccc(Cl)cc3ccn2c1CN(C)C>C(C)O>Cc1nc2c3ccc(Cl)cc3ccn2c1C[N+](C)(C)C.[I-]
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-0f6d18779fe14bc4b673be47f8748154
Cc1nc2c3ccccc3ccn2c1C[N+](C)(C)C.c1c[nH]cn1>>Cc1nc2c3ccccc3ccn2c1Cc1ncc[nH]1
COS(=O)(=O)[O-].CC=1N=C2N(C=CC3=CC=CC=C23)C1C[N+](C)(C)C.N1C=NC=C1>>N1C(=NC=C1)CC1=C(N=C2N1C=CC1=CC=CC=C21)C
C[N+](C)(C)[CH2:15][c:14]1[c:2]([CH3:1])[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][cH:9][c:10]3[cH:11][cH:12][n:13]21.[cH:16]1[n:17][cH:18][cH:19][nH:20]1>>[CH3:1][c:2]1[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][cH:9][c:10]3[cH:11][cH:12][n:13]2[c:14]1[CH2:15][c:16]1[n:17][cH:18][cH:19][nH:20]1
Cc1nc2c3ccccc3ccn2c1C[N+](C)(C)C.c1c[nH]cn1
Cc1nc2c3ccccc3ccn2c1Cc1ncc[nH]1
null
null
C(C)O
C-C Coupling
OtherReaction
1ab3da90f58e99b3fa575495e50a72ec8bd1a302aac79a5abf60bcbe0f90c405
410ec9b1cc243569e4ff568c248f0b402403802e002b4018f576af3f6960507b
c1ccc2c(c1)ccn1c(Cc3ncc[nH]3)cnc21
C-[N+](-C)(-C)-[CH2;D2;+0:1]-[c:2]1:[#7;a:3](:[c:4]):[c:5]:[#7;a:6]:[c:7]:1-[C;D1;H3:8].[#7;a:9]1:[c:10]:[c:11]:[#7;a:12]:[cH;D2;+0:13]:1>>[C;D1;H3:8]-[c:7]1:[#7;a:6]:[c:5]:[#7;a:3](:[c:4]):[c:2]:1-[CH2;D2;+0:1]-[c;H0;D3;+0:13]1:[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:1
71.2
[{"value": 71.2, "product": "N1C(=NC=C1)CC1=C(N=C2N1C=CC1=CC=CC=C21)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
7
HOUR
A mixture of 2-methyl-3-trimethylammoniomethylimidazo[2,1-a]isoquinoline methylsulfate (4.5 g) and imidazole (2.02 g) in ethanol (45 ml) was refluxed with stirring for 7 hours and evaporated in vacuo. To the residue was added water and the resulting precipitates were collected by filtration and recrystallized from a mi...
10.6084/m9.figshare.5104873.v1
null
null
null
c1c[nH]cn1
c1c[nH]cn1
c1ccc2c(c1)ccn1ccnc21.c1c[nH]cn1
Other
C(C)O
null
7
Cc1nc2c3ccccc3ccn2c1C[N+](C)(C)C.c1c[nH]cn1>C(C)O>Cc1nc2c3ccccc3ccn2c1Cc1ncc[nH]1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-f12ff83f9eeb42828ee17781af946cd5
Cc1nc2c3ccccc3ccn2c1C[N+](C)(C)C.Cc1ncc[nH]1>>Cc1nc2c3ccccc3ccn2c1CC1(C)N=CC=N1
COS(=O)(=O)[O-].CC=1N=C2N(C=CC3=CC=CC=C23)C1C[N+](C)(C)C.CC=1NC=CN1>>CC=1N=C2N(C=CC3=CC=CC=C23)C1CC1(N=CC=N1)C
C[N+](C)(C)[CH2:15][c:14]1[c:2]([CH3:1])[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][cH:9][c:10]3[cH:11][cH:12][n:13]21.[c:16]1([CH3:17])[n:18][cH:19][cH:20][nH:21]1>>[CH3:1][c:2]1[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][cH:9][c:10]3[cH:11][cH:12][n:13]2[c:14]1[CH2:15][C:16]1([CH3:17])[N:18]=[CH:19][CH:20]=[N:21]1
Cc1nc2c3ccccc3ccn2c1C[N+](C)(C)C.Cc1ncc[nH]1
Cc1nc2c3ccccc3ccn2c1CC1(C)N=CC=N1
null
null
C(C)O
C-C Coupling
OtherReaction
6c285af82090e6b98ef89274178823fb4d2c97d2095bafb6d419249fc6f7f7c0
184f7d80dc0b974754f7d3970e9cf720d01c801e7b1a9c0474e0cce2fbfd0bb9
C1=NC(Cc2cnc3c4ccccc4ccn23)N=C1
C-[N+](-C)(-C)-[CH2;D2;+0:1]-[c:2]1:[#7;a:3](:[c:4]):[c:5]:[#7;a:6]:[c:7]:1-[C;D1;H3:8].[C;D1;H3:9]-[c;H0;D3;+0:10]1:[n;H0;D2;+0:11]:[cH;D2;+0:12]:[cH;D2;+0:13]:[nH;D2;+0:14]:1>>[C;D1;H3:9]-[C;H0;D4;+0:10]1(-[CH2;D2;+0:1]-[c:2]2:[#7;a:3](:[c:4]):[c:5]:[#7;a:6]:[c:7]:2-[C;D1;H3:8])-[N;H0;D2;+0:11]=[CH;D2;+0:12]-[CH;D2;+...
37.5
[{"value": 37.5, "product": "CC=1N=C2N(C=CC3=CC=CC=C23)C1CC1(N=CC=N1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
A mixture of 2-methyl-3-trimethylammoniomethylimidazo[2,1-a]isoquinoline methylsulfate (3 g) and 2-methylimidazole (1.6 g) in ethanol (50 ml) was refluxed with stirring for 4 hours and evaporated in vacuo. To the residue was added water and the resulting precipitates were collected by filtration, dried and recrystalliz...
10.6084/m9.figshare.5104873.v1
null
null
Substituted imine.Substituted imine
c1c[nH]cn1
C1=NCN=C1
c1ccc2c(c1)ccn1ccnc21.C1=NCN=C1
Other
C(C)O
null
4
Cc1nc2c3ccccc3ccn2c1C[N+](C)(C)C.Cc1ncc[nH]1>C(C)O>Cc1nc2c3ccccc3ccn2c1CC1(C)N=CC=N1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-5cf67d07029a4e36b2dd22857e9ca32e
Cc1nc2c3cccc(Cl)c3ccn2c1C[N+](C)(C)C.c1c[nH]cn1>>Cc1nc2c3cccc(Cl)c3ccn2c1Cc1ncc[nH]1
C(C)O.COS(=O)(=O)[O-].ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3C[N+](C)(C)C)C.N1C=NC=C1>>ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3CC=3NC=CN3)C
C[N+](C)(C)[CH2:16][c:15]1[c:2]([CH3:1])[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][c:9]([Cl:10])[c:11]3[cH:12][cH:13][n:14]21.[cH:17]1[n:18][cH:19][cH:20][nH:21]1>>[CH3:1][c:2]1[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][c:9]([Cl:10])[c:11]3[cH:12][cH:13][n:14]2[c:15]1[CH2:16][c:17]1[n:18][cH:19][cH:20][nH:21]1
Cc1nc2c3cccc(Cl)c3ccn2c1C[N+](C)(C)C.c1c[nH]cn1
Cc1nc2c3cccc(Cl)c3ccn2c1Cc1ncc[nH]1
null
null
CS(=O)C
C-C Coupling
OtherReaction
1ab3da90f58e99b3fa575495e50a72ec8bd1a302aac79a5abf60bcbe0f90c405
410ec9b1cc243569e4ff568c248f0b402403802e002b4018f576af3f6960507b
c1ccc2c(c1)ccn1c(Cc3ncc[nH]3)cnc21
C-[N+](-C)(-C)-[CH2;D2;+0:1]-[c:2]1:[#7;a:3](:[c:4]):[c:5]:[#7;a:6]:[c:7]:1-[C;D1;H3:8].[#7;a:9]1:[c:10]:[c:11]:[#7;a:12]:[cH;D2;+0:13]:1>>[C;D1;H3:8]-[c:7]1:[#7;a:6]:[c:5]:[#7;a:3](:[c:4]):[c:2]:1-[CH2;D2;+0:1]-[c;H0;D3;+0:13]1:[#7;a:9]:[c:10]:[c:11]:[#7;a:12]:1
41
[{"value": 41.0, "product": "ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3CC=3NC=CN3)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
5
HOUR
Ethanol (50 ml) was added to a mixture of 7-chloro-2-methyl-3-trimethylammoniomethylimidazo[2,1-a]isoquinoline methylsulfate (2.3 g) and imidazole (0.95 g) in dimethyl sulfoxide (20 ml) and heated at 100° C. with stirring for 5 hours. After the removal of ethanol by distillation, the residue was poured into water. The ...
10.6084/m9.figshare.5104873.v1
null
null
null
c1c[nH]cn1
c1c[nH]cn1
c1ccc2c(c1)ccn1ccnc21.c1c[nH]cn1
Other
CS(=O)C
100
5
Cc1nc2c3cccc(Cl)c3ccn2c1C[N+](C)(C)C.c1c[nH]cn1>CS(=O)C>Cc1nc2c3cccc(Cl)c3ccn2c1Cc1ncc[nH]1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-9ea9b772f2ac449680941eb9538ee16f
Cc1nc2c3ccccc3ccn2c1CC#N.[N-]=[N+]=[N-]>>Cc1nc2c3ccccc3ccn2c1Cc1nnn[nH]1
Cl.C(#N)CC1=C(N=C2N1C=CC1=CC=CC=C21)C.[Cl-].[NH4+].[N-]=[N+]=[N-].[Na+].C([O-])(O)=O.[Na+]>>CC=1N=C2N(C=CC3=CC=CC=C23)C1CC1=NN=NN1
[CH3:1][c:2]1[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][cH:9][c:10]3[cH:11][cH:12][n:13]2[c:14]1[CH2:15][C:16]#[N:17].[N-:18]=[N+:19]=[N-:20]>>[CH3:1][c:2]1[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][cH:9][c:10]3[cH:11][cH:12][n:13]2[c:14]1[CH2:15][c:16]1[n:17][n:18][n:19][nH:20]1
Cc1nc2c3ccccc3ccn2c1CC#N.[N-]=[N+]=[N-]
Cc1nc2c3ccccc3ccn2c1Cc1nnn[nH]1
null
null
O.CN(C=O)C
Aromatic Heterocycle Formation
OtherReaction
237b84aaa459abf427f233dc6a07a1d9de824f980714e458423189bb68f60f12
d8c808528b7ee68720aaeebd35cb6a2a30e344748d0066102cdae99843b93cf0
c1ccc2c(c1)ccn1c(Cc3nnn[nH]3)cnc21
[#7;a:1]:[c:2](-[C:3]-[C;H0;D2;+0:4]#[N;H0;D1;+0:5]):[c:6]:[#7;a:7].[N-;H0;D1:8]=[N+;H0;D2:9]=[N-;H0;D1:10]>>[#7;a:1]:[c:2](-[C:3]-[c;H0;D3;+0:4]1:[n;H0;D2;+0:5]:[n;H0;D2;+0:8]:[n;H0;D2;+0:9]:[nH;D2;+0:10]:1):[c:6]:[#7;a:7]
86.7
[{"value": 86.7, "product": "CC=1N=C2N(C=CC3=CC=CC=C23)C1CC1=NN=NN1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
18
HOUR
A mixture of 3-cyanomethyl-2-methylimidazo[2,1-a]isoquinoline (2.8 g), ammonium chloride (0.74 g) and sodium azide (0.9 g) in N,N-dimethylformamide (28 ml) was heated at 120°-125° C. with stirring for 18 hours. The solution was poured into water, acidified with concentrated hydrochloric acid and then neutralized with a...
10.6084/m9.figshare.5104873.v1
null
Nitrile
null
null
c1nnn[nH]1
c1ccc2c(c1)ccn1ccnc21.c1nnn[nH]1
null
O.CN(C=O)C
null
18
Cc1nc2c3ccccc3ccn2c1CC#N.[N-]=[N+]=[N-]>O.CN(C=O)C>Cc1nc2c3ccccc3ccn2c1Cc1nnn[nH]1
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-cb697b53c8a94fa7a4450949dd32dd23
CN(C)C=O.Cc1cn2ccc3c(Cl)cccc3c2n1>>Cc1nc2c3cccc(Cl)c3ccn2c1C=O
[OH-].[Na+].ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3)C.P(=O)(Cl)(Cl)Cl.CN(C=O)C.CN(C=O)C>>ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3C=O)C
CN(C)[CH:16]=[O:17].[CH3:1][c:2]1[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][c:9]([Cl:10])[c:11]3[cH:12][cH:13][n:14]2[cH:15]1>>[CH3:1][c:2]1[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][c:9]([Cl:10])[c:11]3[cH:12][cH:13][n:14]2[c:15]1[CH:16]=[O:17]
CN(C)C=O.Cc1cn2ccc3c(Cl)cccc3c2n1
Cc1nc2c3cccc(Cl)c3ccn2c1C=O
null
null
null
C-C Coupling
OtherReaction
d5c314a91dcd787871cba8969054bfc3edcf395cb9c2c24e493337f14c07a0da
f0bd75a0630092c31f21f61f4a015c77ae0dff14a0b742b4370d7a38fda490f7
c1ccc2c(c1)ccn1ccnc21
C-N(-C)-[CH;D2;+0:1]=[O;D1;H0:2].[C;D1;H3:3]-[c:4]1:[#7;a:5]:[c:6](:[c:7]):[#7;a:8](:[c:9]):[cH;D2;+0:10]:1>>[C;D1;H3:3]-[c:4]1:[#7;a:5]:[c:6](:[c:7]):[#7;a:8](:[c:9]):[c;H0;D3;+0:10]:1-[CH;D2;+0:1]=[O;D1;H0:2]
null
[]
80
CELSIUS
6
HOUR
A solution of 7-chloro-2-methylimidazo[2,1-a]isoquinoline (4 g) in N,N-dimethylformamide (40 ml) was added dropwise to a mixture of N,N-dimethylformamide (5.7 ml) and phosphoryl chloride (1.86 ml) under ice cooling. After being stirred at 85°-90° C. for 6 hours, the mixture was poured into ice-water, basified with aque...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide
Aldehyde
c1ccc2c(c1)ccn1ccnc21
c1ccc2c(c1)ccn1ccnc21
c1ccc2c(c1)ccn1ccnc21
Other
null
80
6
CN(C)C=O.Cc1cn2ccc3c(Cl)cccc3c2n1>>Cc1nc2c3cccc(Cl)c3ccn2c1C=O
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-bad33391a14d457ea99c0d986f93938b
CC(C)CCON=O.Cc1cn2ccc3c(Cl)cccc3c2n1>>Cc1nc2c3cccc(Cl)c3ccn2c1N=O
N(=O)OCCC(C)C.ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3)C>>ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3N=O)C
CC(C)CCO[N:16]=[O:17].[CH3:1][c:2]1[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][c:9]([Cl:10])[c:11]3[cH:12][cH:13][n:14]2[cH:15]1>>[CH3:1][c:2]1[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][c:9]([Cl:10])[c:11]3[cH:12][cH:13][n:14]2[c:15]1[N:16]=[O:17]
CC(C)CCON=O.Cc1cn2ccc3c(Cl)cccc3c2n1
Cc1nc2c3cccc(Cl)c3ccn2c1N=O
null
null
O1CCOCC1
Heteroatom Alkylation and Arylation
OtherReaction
8a9a27bda14d96d3b7c1d80813b1121948071de1e7bcc58c0b006d6d878ebee4
cf1232fd5519ec578bdba0cee2907500a1299052406ff82030a98b4dcbee91ea
c1ccc2c(c1)ccn1ccnc21
C-C(-C)-C-C-O-[N;H0;D2;+0:1]=[O;D1;H0:2].[C;D1;H3:3]-[c:4]1:[#7;a:5]:[c:6](:[c:7]):[#7;a:8](:[c:9]):[cH;D2;+0:10]:1>>[C;D1;H3:3]-[c:4]1:[#7;a:5]:[c:6](:[c:7]):[#7;a:8](:[c:9]):[c;H0;D3;+0:10]:1-[N;H0;D2;+0:1]=[O;D1;H0:2]
39.7
[{"value": 39.7, "product": "ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3N=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Isoamyl nitrite (140 g) was added to a suspension of 7-chloro-2-methylimidazo[2,1-a]isoquinoline (17.1 g) in dioxane (170 ml) at 50° C. and the mixture was refluxed for 15 minutes. After being cooled, the resulting precipitate was collected by filtration, washed successively with dioxane and diethyl ether and dried in ...
10.6084/m9.figshare.5104873.v1
null
Nitroso
Nitroso
c1ccc2c(c1)ccn1ccnc21
c1ccc2c(c1)ccn1ccnc21
c1ccc2c(c1)ccn1ccnc21
HO-
O1CCOCC1
null
null
CC(C)CCON=O.Cc1cn2ccc3c(Cl)cccc3c2n1>O1CCOCC1>Cc1nc2c3cccc(Cl)c3ccn2c1N=O
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-0a9890bc81aa4816a540a63440317a80
Cc1nc2c3cccc(Cl)c3ccn2c1N=O>>Cc1nc2c3cccc(Cl)c3ccn2c1N
ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3N=O)C.C(C)(=O)O>>NC1=C(N=C2N1C=CC1=C(C=CC=C21)Cl)C
O=[N:16][c:15]1[c:2]([CH3:1])[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][c:9]([Cl:10])[c:11]3[cH:12][cH:13][n:14]21>>[CH3:1][c:2]1[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][c:9]([Cl:10])[c:11]3[cH:12][cH:13][n:14]2[c:15]1[NH2:16]
Cc1nc2c3cccc(Cl)c3ccn2c1N=O
Cc1nc2c3cccc(Cl)c3ccn2c1N
null
[Zn]
O
Reduction
OtherReaction
10bd501bc4fc8c6849398545fc18bd5f6b51ea4e37b15a00157d17550a6b88bf
7085a0cec3cc6daaf2fab855d070c407558563b5b6837070687c0df0a552c6fe
c1ccc2c(c1)ccn1ccnc21
O=[N;H0;D2;+0:1]-[c:2]1:[#7;a:3](:[c:4]):[c:5]:[#7;a:6]:[c:7]:1-[C;D1;H3:8]>>[C;D1;H3:8]-[c:7]1:[#7;a:6]:[c:5]:[#7;a:3](:[c:4]):[c:2]:1-[NH2;D1;+0:1]
80.6
[{"value": 80.6, "product": "NC1=C(N=C2N1C=CC1=C(C=CC=C21)Cl)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Zinc powder (10.2 g) was added portionwise to a mixture of 7-chloro-2-methyl-3-nitrosoimidazo[2,1-a]isoquinoline (7.7 g) and acetic acid (100 ml) in water (77 ml) over a period of 7 hours and then the mixture was filtered by suction. The filtrate was evaporated in vacuo and the residue was extracted with chloroform aft...
10.6084/m9.figshare.5104873.v1
null
Nitroso
Primary amine
null
null
c1ccc2c(c1)ccn1ccnc21
Other
[Zn].O
null
null
Cc1nc2c3cccc(Cl)c3ccn2c1N=O>[Zn].O>Cc1nc2c3cccc(Cl)c3ccn2c1N
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-f3890f0223094eaf9a2ee3e8c44021d2
CCOC=NC#N.Cc1nc2c3cccc(Cl)c3ccn2c1N>>Cc1nc2c3cccc(Cl)c3ccn2c1N=CNC#N
C(#N)N=COCC.NC1=C(N=C2N1C=CC1=C(C=CC=C21)Cl)C>>C(#N)NC=NC1=C(N=C2N1C=CC1=C(C=CC=C21)Cl)C
CCO[CH:17]=[N:18][C:19]#[N:20].[CH3:1][c:2]1[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][c:9]([Cl:10])[c:11]3[cH:12][cH:13][n:14]2[c:15]1[NH2:16]>>[CH3:1][c:2]1[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][c:9]([Cl:10])[c:11]3[cH:12][cH:13][n:14]2[c:15]1[N:16]=[CH:17][NH:18][C:19]#[N:20]
CCOC=NC#N.Cc1nc2c3cccc(Cl)c3ccn2c1N
Cc1nc2c3cccc(Cl)c3ccn2c1N=CNC#N
null
null
C(C)O
Heteroatom Alkylation and Arylation
OtherReaction
a37366ff71575f45a48ed3e6fbcb7aa2756c4f130276f97e7773c1fa36ecb300
500f5fcf4fe90cec5c76ba5467901dd2145f02581496325c98a098ab95a67794
c1ccc2c(c1)ccn1ccnc21
C-C-O-[CH;D2;+0:1]=[N;H0;D2;+0:2]-[C:3]#[N;D1;H0:4].[C;D1;H3:5]-[c:6]1:[#7;a:7]:[c:8]:[#7;a:9](:[c:10]):[c:11]:1-[NH2;D1;+0:12]>>[C;D1;H3:5]-[c:6]1:[#7;a:7]:[c:8]:[#7;a:9](:[c:10]):[c:11]:1-[N;H0;D2;+0:12]=[CH;D2;+0:1]-[NH;D2;+0:2]-[C:3]#[N;D1;H0:4]
35.5
[{"value": 35.5, "product": "C(#N)NC=NC1=C(N=C2N1C=CC1=C(C=CC=C21)Cl)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
45
HOUR
Ethyl N-cyanoformimidate (3.2 g) was added to a suspension of 3-amino-7-chloro-2-methylimidazo[2,1-a]isoquinoline (2.3 g) in ethanol (60 ml) and the mixture was stirred at room temperature for 45 hours. The mixture was evaporated in vacuo and the residual solid was washed successively with diethyl ether and ethyl aceta...
10.6084/m9.figshare.5104873.v1
null
Ether.Primary amine
Cyanamide
null
null
c1ccc2c(c1)ccn1ccnc21
HO-
C(C)O
null
45
CCOC=NC#N.Cc1nc2c3cccc(Cl)c3ccn2c1N>C(C)O>Cc1nc2c3cccc(Cl)c3ccn2c1N=CNC#N
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-a2572d18a38f4d67add05b3833facf30
Cc1nc2c3cccc(Cl)c3ccn2c1CSCCN.O=S1(=O)N=C(Cl)c2ccccc21>>Cc1nc2c3cccc(Cl)c3ccn2c1CSCCNC1=NS(=O)(=O)c2ccccc21
NCCSCC1=C(N=C2N1C=CC1=C(C=CC=C21)Cl)C.C(C)N(CC)CC.ClC1=NS(C2=C1C=CC=C2)(=O)=O>>ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3CSCCNC3=NS(C1=C3C=CC=C1)(=O)=O)C
[CH3:1][c:2]1[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][c:9]([Cl:10])[c:11]3[cH:12][cH:13][n:14]2[c:15]1[CH2:16][S:17][CH2:18][CH2:19][NH2:20].Cl[C:21]1=[N:22][S:23](=[O:24])(=[O:25])[c:26]2[cH:27][cH:28][cH:29][cH:30][c:31]21>>[CH3:1][c:2]1[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][c:9]([Cl:10])[c:11]3[cH:12][cH:13][n:14]2[c:15]1[C...
Cc1nc2c3cccc(Cl)c3ccn2c1CSCCN.O=S1(=O)N=C(Cl)c2ccccc21
Cc1nc2c3cccc(Cl)c3ccn2c1CSCCNC1=NS(=O)(=O)c2ccccc21
null
null
C(C)O
Heteroatom Alkylation and Arylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_N
8199fc5915162236b20d33826bdc3127d185693d629514b69e969b9e767eacd2
c0f977b53197d39fa813083b5189dbda6c3d3288d4a3f9a6de603ab0d69db97f
O=S1(=O)N=C(NCCSCc2cnc3c4ccccc4ccn23)c2ccccc21
Cl-[C;H0;D3;+0:1]1=[#7:2]-[#16:3]-[c:4]:[c:5]-1:[c:6].[C:7]-[C:8]-[NH2;D1;+0:9]>>[C:7]-[C:8]-[NH;D2;+0:9]-[C;H0;D3;+0:1]1=[#7:2]-[#16:3]-[c:4]:[c:5]-1:[c:6]
95.2
[{"value": 95.2, "product": "ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3CSCCNC3=NS(C1=C3C=CC=C1)(=O)=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a mixture of 3-(2-aminoethyl)thiomethyl-7-chloro-2-methylimidazo[2,1-a]isoquinoline (1.5 g) and triethylamine (0.5 g) in ethyl alcohol (35 ml) was added portionwise 3-chloro-1,2-benzisothiazole-1,1dioxide (1.0 g). After being stirred at ambient temperature for 1 hour, the resulting precipitate was collected by filtr...
10.6084/m9.figshare.5104873.v1
null
Alkenyl halide.Primary amine
Secondary amine
c1ccc2sncc2c1
c1ccc2sncc2c1
c1ccc2c(c1)ccn1ccnc21.c1ccc2sncc2c1
HCl
C(C)O
null
1
Cc1nc2c3cccc(Cl)c3ccn2c1CSCCN.O=S1(=O)N=C(Cl)c2ccccc21>C(C)O>Cc1nc2c3cccc(Cl)c3ccn2c1CSCCNC1=NS(=O)(=O)c2ccccc21
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-111a73a408064d02b9746897538f896a
CSCc1c(C)nc2c3cccc(Cl)c3ccn12.O=C(OO)c1cccc(Cl)c1>>Cc1nc2c3cccc(Cl)c3ccn2c1CS(C)=O
ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3CSC)C.ClC1=CC(=CC=C1)C(=O)OO>>ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3CS(=O)C)C
[CH3:1][c:2]1[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][c:9]([Cl:10])[c:11]3[cH:12][cH:13][n:14]2[c:15]1[CH2:16][S:17][CH3:18].O=C(O[OH:19])c1cccc(Cl)c1>>[CH3:1][c:2]1[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][c:9]([Cl:10])[c:11]3[cH:12][cH:13][n:14]2[c:15]1[CH2:16][S:17]([CH3:18])=[O:19]
CSCc1c(C)nc2c3cccc(Cl)c3ccn12.O=C(OO)c1cccc(Cl)c1
Cc1nc2c3cccc(Cl)c3ccn2c1CS(C)=O
null
null
C(Cl)(Cl)Cl
Oxidation
Sulfanyl to sulfinyl_peroxide
95b5106b07a173d8eafc1c9c8a6c938befe131c3d1caaf5886529b7aee55ea9d
7652b53bb02130dccfe4b1e8905d7f3db7f05ff3a95a0003c1bab09b1ad4083e
c1ccc2c(c1)ccn1ccnc21
Cl-c1:c:c:c:c(-C(=O)-O-[OH;D1;+0:1]):c:1.[#7;a:2]:[c:3](-[C:4]-[S;H0;D2;+0:5]-[C;D1;H3:6]):[c:7]:[#7;a:8]>>[#7;a:2]:[c:3](-[C:4]-[S;H0;D3;+0:5](-[C;D1;H3:6])=[O;H0;D1;+0:1]):[c:7]:[#7;a:8]
64.3
[{"value": 64.3, "product": "ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3CS(=O)C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
To a solution of 7-chloro-2-methyl-3-methylthiomethylimidazo[2,1-a]isoquinoline (2 g) in chloroform (20 ml) was added portionwise 70% m-chloroperbenzoic acid (1.78 g). After being stirred under ice cooling for 30 minutes, the mixture was washed successively with aqueous sodium bicarbonate, water and brine, dried over m...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Peroxide.Monosulfide
Sulfoxide
c1ccccc1
null
c1ccc2c(c1)ccn1ccnc21
HCl
C(Cl)(Cl)Cl
null
0.5
CSCc1c(C)nc2c3cccc(Cl)c3ccn12.O=C(OO)c1cccc(Cl)c1>C(Cl)(Cl)Cl>Cc1nc2c3cccc(Cl)c3ccn2c1CS(C)=O
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-8d9ad75ce0ee48ae823f1d493e44156c
CCOC(=O)Cc1c(C)nc2c3cccc(Cl)c3ccn12>>Cc1nc2c3cccc(Cl)c3ccn2c1CC(=O)O
[OH-].[Na+].ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3CC(=O)OCC)C.CO>>C(=O)(O)CC1=C(N=C2N1C=CC1=C(C=CC=C21)Cl)C
CC[O:19][C:17]([CH2:16][c:15]1[c:2]([CH3:1])[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][c:9]([Cl:10])[c:11]3[cH:12][cH:13][n:14]21)=[O:18]>>[CH3:1][c:2]1[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][c:9]([Cl:10])[c:11]3[cH:12][cH:13][n:14]2[c:15]1[CH2:16][C:17](=[O:18])[OH:19]
CCOC(=O)Cc1c(C)nc2c3cccc(Cl)c3ccn12
Cc1nc2c3cccc(Cl)c3ccn2c1CC(=O)O
null
null
O
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc2c(c1)ccn1ccnc21
C-C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
74.2
[{"value": 74.2, "product": "C(=O)(O)CC1=C(N=C2N1C=CC1=C(C=CC=C21)Cl)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of sodium hydroxide (1.25 g) in water (5 ml) was added to a mixture of 7-chloro-3-ethoxycarbonylmethyl-2-methylimidazo[2,1-a]isoquinoline (4.75 g) and methanol (48 ml) and the mixture was refluxed for 1.5 hours. After being cooled, the mixture was evaporated in vacuo and 1N hydrochloric acid (31.4 ml) was ad...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccc2c(c1)ccn1ccnc21
Other
O
null
null
CCOC(=O)Cc1c(C)nc2c3cccc(Cl)c3ccn12>O>Cc1nc2c3cccc(Cl)c3ccn2c1CC(=O)O
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-5862c7b217584878baaa24553651cf1a
Cc1nc2c3cccc(Cl)c3ccn2c1C(=O)O.O=S(Cl)Cl>>Cc1nc2c3cccc(Cl)c3ccn2c1C(=O)Cl.Cl
C(=O)(O)C1=C(N=C2N1C=CC1=C(C=CC=C21)Cl)C.S(=O)(Cl)Cl>>Cl.ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3C(=O)Cl)C
O[C:16]([c:15]1[c:2]([CH3:1])[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][c:9]([Cl:10])[c:11]3[cH:12][cH:13][n:14]21)=[O:17].O=S([Cl:18])[Cl:19]>>[CH3:1][c:2]1[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][c:9]([Cl:10])[c:11]3[cH:12][cH:13][n:14]2[c:15]1[C:16](=[O:17])[Cl:18].[ClH:19]
Cc1nc2c3cccc(Cl)c3ccn2c1C(=O)O.O=S(Cl)Cl
Cc1nc2c3cccc(Cl)c3ccn2c1C(=O)Cl.Cl
null
null
null
Functional Group Interconversion
Alcohol to chloride_SOCl2
c301c14a9dcd0670d52e8b77396cbe7fd8edeedd757bc43f4162ade1fc52fc93
787f545db5dc0b29dde55b5fbed7db8625b8055f49327f97ed4d83cc47c3af1d
c1ccc2c(c1)ccn1ccnc21
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#7;a:4](:[c:5]):[c:6]:[#7;a:7]:[c:8]:1-[C;D1;H3:9].O=S(-[Cl;H0;D1;+0:10])-[Cl;H0;D1;+0:11]>>[C;D1;H3:9]-[c:8]1:[#7;a:7]:[c:6]:[#7;a:4](:[c:5]):[c:3]:1-[C;H0;D3;+0:1](-[Cl;H0;D1;+0:10])=[O;D1;H0:2].[ClH;D0;+0:11]
null
[]
null
null
null
null
A mixture of 3-carboxy-7-chloro-2-methylimidazo[2,1-a]isoquinoline (2.5 g) and thionyl chloride (20 ml) was refluxed for 1 hour and evaporated in vacuo. The residual solid was washed with benzene and dried in a desiccator to give 7-chloro-3-chloroformyl-2-methylimidazo[2,1-a]isoquinoline hydrochloride (2.75 g). Conditi...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Acyl halide
null
null
c1ccc2c(c1)ccn1ccnc21
Other
null
null
null
Cc1nc2c3cccc(Cl)c3ccn2c1C(=O)O.O=S(Cl)Cl>>Cc1nc2c3cccc(Cl)c3ccn2c1C(=O)Cl.Cl
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-723db561936c4818afb8fb304b155dd1
Cc1nc2c3cccc(Cl)c3ccn2c1C(=O)Cl.[NH4+]>>Cc1nc2c3cccc(Cl)c3ccn2c1C(N)=O
Cl.ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3C(=O)Cl)C.[OH-].[NH4+]>>C(N)(=O)C1=C(N=C2N1C=CC1=C(C=CC=C21)Cl)C
Cl[C:16]([c:15]1[c:2]([CH3:1])[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][c:9]([Cl:10])[c:11]3[cH:12][cH:13][n:14]21)=[O:18].[NH4+:17]>>[CH3:1][c:2]1[n:3][c:4]2[c:5]3[cH:6][cH:7][cH:8][c:9]([Cl:10])[c:11]3[cH:12][cH:13][n:14]2[c:15]1[C:16]([NH2:17])=[O:18]
Cc1nc2c3cccc(Cl)c3ccn2c1C(=O)Cl.[NH4+]
Cc1nc2c3cccc(Cl)c3ccn2c1C(N)=O
null
null
null
Acylation
OtherReaction
825fddffa01c850bd0103537ce4e244cb6de8bd215cd5da035957375af67e2c9
8805c6321825cef45671bed501723a033e52ab76593d6f4fb97580f38c5af25f
c1ccc2c(c1)ccn1ccnc21
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#7;a:4](:[c:5]):[c:6]:[#7;a:7]:[c:8]:1-[C;D1;H3:9].[NH4+;D0:10]>>[C;D1;H3:9]-[c:8]1:[#7;a:7]:[c:6]:[#7;a:4](:[c:5]):[c:3]:1-[C;H0;D3;+0:1](-[NH2;D1;+0:10])=[O;D1;H0:2]
null
[]
null
null
null
null
To 28% ammonium hydroxide (50 ml) was added 7-chloro-3-chloroformyl-2-methylimidazo[2,1-a]isoquinoline hydrochloride (1.3 g) and the mixture was stirred under ice-cooling for 40 minutes. The resulting precipitate was collected by filtration, washed with water and recrystallized from a mixture of chloroform and methanol...
10.6084/m9.figshare.5104873.v1
null
Acyl halide
Primary amide
null
null
c1ccc2c(c1)ccn1ccnc21
HCl
null
null
null
Cc1nc2c3cccc(Cl)c3ccn2c1C(=O)Cl.[NH4+]>>Cc1nc2c3cccc(Cl)c3ccn2c1C(N)=O
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-1dc58f9bdebb49a9ac8f93e49b2889db
CC(=O)OC(C)=O.Cc1nc2c3cccc(Cl)c3ccn2c1CO>>CC(=O)OCc1c(C)nc2c3cccc(Cl)c3ccn12
C(C)(=O)OC(C)=O.ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3CO)C>>C(C)(=O)OCC1=C(N=C2N1C=CC1=C(C=CC=C21)Cl)C
CC(=O)O[C:2]([CH3:1])=[O:3].[OH:4][CH2:5][c:6]1[c:7]([CH3:8])[n:9][c:10]2[c:11]3[cH:12][cH:13][cH:14][c:15]([Cl:16])[c:17]3[cH:18][cH:19][n:20]12>>[CH3:1][C:2](=[O:3])[O:4][CH2:5][c:6]1[c:7]([CH3:8])[n:9][c:10]2[c:11]3[cH:12][cH:13][cH:14][c:15]([Cl:16])[c:17]3[cH:18][cH:19][n:20]12
CC(=O)OC(C)=O.Cc1nc2c3cccc(Cl)c3ccn2c1CO
CC(=O)OCc1c(C)nc2c3cccc(Cl)c3ccn12
null
null
N1=CC=CC=C1
Acylation
Transesterification
f81e513b7b512b10157c16426844efd8d88e34c97987c1347c6ba8a688351205
fc27d67c790d5fb520ba5d49de1490661fa5b822b714863734ce7e3029dfa84f
c1ccc2c(c1)ccn1ccnc21
C-C(=O)-O-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[#7;a:4]:[c:5](-[C:6]-[OH;D1;+0:7]):[c:8]:[#7;a:9]>>[#7;a:4]:[c:5](-[C:6]-[O;H0;D2;+0:7]-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3]):[c:8]:[#7;a:9]
35.8
[{"value": 35.8, "product": "C(C)(=O)OCC1=C(N=C2N1C=CC1=C(C=CC=C21)Cl)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
24
HOUR
Acetic anhydride (0.71 g) was added dropwise to a suspension of 7-chloro-3-hydroxymethyl-2-methylimidazo[2,1-a]isoquinoline (1.43 g) in pyridine (14 ml) and the mixture was stirred at room temperature for 24 hours. The mixture was evaporated in vacuo and the residue was extracted with chloroform after an addition of wa...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Primary alcohol
Ester
null
null
c1ccc2c(c1)ccn1ccnc21
HO-
N1=CC=CC=C1
null
24
CC(=O)OC(C)=O.Cc1nc2c3cccc(Cl)c3ccn2c1CO>N1=CC=CC=C1>CC(=O)OCc1c(C)nc2c3cccc(Cl)c3ccn12
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-42b24e713fe94be38ed0e09db8750803
CCOC(=O)C(Br)C(C)=O.Nc1nccc2c(Cl)cccc12>>CCOC(=O)c1c(C)nc2c3cccc(Cl)c3ccn12
NC1=NC=CC2=C(C=CC=C12)Cl.C(C)(=O)C(C(=O)OCC)Br.C([O-])(O)=O.[Na+]>>ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3C(=O)OCC)C
O=[C:7]([CH:6](Br)[C:4]([O:3][CH2:2][CH3:1])=[O:5])[CH3:8].[NH2:9][c:10]1[c:11]2[cH:12][cH:13][cH:14][c:15]([Cl:16])[c:17]2[cH:18][cH:19][n:20]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[c:7]([CH3:8])[n:9][c:10]2[c:11]3[cH:12][cH:13][cH:14][c:15]([Cl:16])[c:17]3[cH:18][cH:19][n:20]12
CCOC(=O)C(Br)C(C)=O.Nc1nccc2c(Cl)cccc12
CCOC(=O)c1c(C)nc2c3cccc(Cl)c3ccn12
null
null
C(C)O
Aromatic Heterocycle Formation
OtherReaction
9291871536236f56f37949a16a753eb2f668aa620f1e00d8b8b579b532f4d373
31aa25659cf5accd41f8ff85a49e4d2b829110bf1926ff7161f2261cc71e0db2
c1ccc2c(c1)ccn1ccnc21
Br-[CH;D3;+0:1](-[C:2](=[O;D1;H0:3])-[#8:4]-[C:5])-[C;H0;D3;+0:6](=O)-[C;D1;H3:7].[NH2;D1;+0:8]-[c:9](:[c:10]):[n;H0;D2;+0:11]:[c:12]:[c:13]>>[C:5]-[#8:4]-[C:2](=[O;D1;H0:3])-[c;H0;D3;+0:1]1:[c;H0;D3;+0:6](-[C;D1;H3:7]):[n;H0;D2;+0:8]:[c:9](:[c:10]):[n;H0;D3;+0:11]:1:[c:12]:[c:13]
59.1
[{"value": 59.1, "product": "ClC1=C2C=CN3C(C2=CC=C1)=NC(=C3C(=O)OCC)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 1-amino-5-chloroisoquinoline (6.1 g), ethyl 2-acetyl-2-bromoacetate (10.75 g) and sodium bicarbonate (14.36 g) in ethanol (72 ml) was refluxed for 2 hours and then filtered by suction. The filtrate was evaporated in vacuo, and the residue was dissolved in a mixture of chloroform and methanol. The solution ...
10.6084/m9.figshare.5104873.v1
null
Secondary halide.Ketone.Ester.Primary amine
Ester
c1ccc2cnccc2c1
c1ccc2c(c1)ccn1ccnc21
c1ccc2c(c1)ccn1ccnc21
HBr
C(C)O
null
null
CCOC(=O)C(Br)C(C)=O.Nc1nccc2c(Cl)cccc12>C(C)O>CCOC(=O)c1c(C)nc2c3cccc(Cl)c3ccn12
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-ede232d689f540df962a4f077637f4cb
CC(=O)C(Cl)C(C)=O.Nc1nccc2c(Cl)cccc12>>CC(=O)c1c(C)nc2c3cccc(Cl)c3ccn12
NC1=NC=CC2=C(C=CC=C12)Cl.ClC(C(C)=O)C(C)=O>>C(C)(=O)C1=C(N=C2N1C=CC1=C(C=CC=C21)Cl)C
O=[C:5]([CH:4](Cl)[C:2]([CH3:1])=[O:3])[CH3:6].[NH2:7][c:8]1[c:9]2[cH:10][cH:11][cH:12][c:13]([Cl:14])[c:15]2[cH:16][cH:17][n:18]1>>[CH3:1][C:2](=[O:3])[c:4]1[c:5]([CH3:6])[n:7][c:8]2[c:9]3[cH:10][cH:11][cH:12][c:13]([Cl:14])[c:15]3[cH:16][cH:17][n:18]12
CC(=O)C(Cl)C(C)=O.Nc1nccc2c(Cl)cccc12
CC(=O)c1c(C)nc2c3cccc(Cl)c3ccn12
null
null
C(Cl)(Cl)Cl
Aromatic Heterocycle Formation
OtherReaction
9f0f2feb819af86b589d5040ae3a0e6b5661f8a161cc2164158df119601b38b0
bcfaaca1fff120fc45a5fcf802a81a9be77560ebe832f4ae204a887e33863aca
c1ccc2c(c1)ccn1ccnc21
Cl-[CH;D3;+0:1](-[C:2](-[C;D1;H3:3])=[O;D1;H0:4])-[C;H0;D3;+0:5](=O)-[C;D1;H3:6].[NH2;D1;+0:7]-[c:8](:[c:9]):[n;H0;D2;+0:10]:[c:11]:[c:12]>>[C;D1;H3:3]-[C:2](=[O;D1;H0:4])-[c;H0;D3;+0:1]1:[c;H0;D3;+0:5](-[C;D1;H3:6]):[n;H0;D2;+0:7]:[c:8](:[c:9]):[n;H0;D3;+0:10]:1:[c:11]:[c:12]
9
[{"value": 9.0, "product": "C(C)(=O)C1=C(N=C2N1C=CC1=C(C=CC=C21)Cl)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a suspension of 1-amino-5-chloroisoquinoline (10 g) in chloroform (150 ml) was added dropwise 3-chloro-2,4-pentanedione (11.3 g). The mixture was refluxed for 6 hours and then allowed to stand at room temperature over night. The mixture was washed successively with aqueous sodium bicarbonate and water, dried over ma...
10.6084/m9.figshare.5104873.v1
null
Secondary halide.Ketone.Ketone.Primary amine
Ketone
c1ccc2cnccc2c1
c1ccc2c(c1)ccn1ccnc21
c1ccc2c(c1)ccn1ccnc21
HCl
C(Cl)(Cl)Cl
null
null
CC(=O)C(Cl)C(C)=O.Nc1nccc2c(Cl)cccc12>C(Cl)(Cl)Cl>CC(=O)c1c(C)nc2c3cccc(Cl)c3ccn12
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-55a62297bd47465797a5e421f0df4cfa
O=C(Cc1ccccc1)N[C@@H]1C(=O)N2C(C(=O)OC(c3ccccc3)c3ccccc3)=C(CO)CS[C@H]12.O=S(Cl)Cl>>O=C(Cc1ccccc1)N[C@@H]1C(=O)N2C(C(=O)OC(c3ccccc3)c3ccccc3)=C(CCl)CS[C@H]12
OCC=1CS[C@H]2N(C1C(=O)OC(C1=CC=CC=C1)C1=CC=CC=C1)C([C@H]2NC(CC2=CC=CC=C2)=O)=O.N1=CC=CC=C1.CN(C=O)C.S(=O)(Cl)Cl>>ClCC=1CS[C@H]2N(C1C(=O)OC(C1=CC=CC=C1)C1=CC=CC=C1)C([C@H]2NC(CC2=CC=CC=C2)=O)=O
O[CH2:33][C:32]1=[C:15]([C:16](=[O:17])[O:18][CH:19]([c:20]2[cH:21][cH:22][cH:23][cH:24][cH:25]2)[c:26]2[cH:27][cH:28][cH:29][cH:30][cH:31]2)[N:14]2[C:12](=[O:13])[C@@H:11]([NH:10][C:2](=[O:1])[CH2:3][c:4]3[cH:5][cH:6][cH:7][cH:8][cH:9]3)[C@H:37]2[S:36][CH2:35]1.O=S(Cl)[Cl:34]>>[O:1]=[C:2]([CH2:3][c:4]1[cH:5][cH:6][cH:...
O=C(Cc1ccccc1)N[C@@H]1C(=O)N2C(C(=O)OC(c3ccccc3)c3ccccc3)=C(CO)CS[C@H]12.O=S(Cl)Cl
O=C(Cc1ccccc1)N[C@@H]1C(=O)N2C(C(=O)OC(c3ccccc3)c3ccccc3)=C(CCl)CS[C@H]12
null
null
O1CCCC1
Functional Group Interconversion
Alcohol to chloride_SOCl2
bb752b9027dc4488ba075e5955118a819f80cabd751a7497b67c2eeb1db6b071
cbf41c7cf9fe6b47a243b1674d74ed5bf46a151f7f3a71d206e23176e158facf
O=C(Cc1ccccc1)N[C@@H]1C(=O)N2C(C(=O)OC(c3ccccc3)c3ccccc3)=CCS[C@H]12
Cl-S(=O)-[Cl;H0;D1;+0:1].O-[CH2;D2;+0:2]-[C:3](=[C:4](-[C:5](-[#8:6])=[O;D1;H0:7])-[#7:8]-[C:9]=[O;D1;H0:10])-[C:11]-[#16:12]>>[#16:12]-[C:11]-[C:3](-[CH2;D2;+0:2]-[Cl;H0;D1;+0:1])=[C:4](-[C:5](-[#8:6])=[O;D1;H0:7])-[#7:8]-[C:9]=[O;D1;H0:10]
null
[]
null
null
10
MINUTE
24 ml (0.3 mole) of pyridine, 400 μl of dimethylformamide and 21.6 ml (0.3 mole) of thionyl chloride are added to a solution of 103 g (0.2 mole) of benzhydryl 3-hydroxymethyl-7β-phenylacetamido-3-cephem-4-carboxylate (prepared, for example, in accordance with Helv. Chim. Acta 57, 2044 (1974)) in 3.5 l of absolute tetra...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Primary halide
null
null
c1ccccc1.c1ccccc1.c1ccccc1.C1=CN2CC[C@H]2SC1
HCl
O1CCCC1
null
0.166667
O=C(Cc1ccccc1)N[C@@H]1C(=O)N2C(C(=O)OC(c3ccccc3)c3ccccc3)=C(CO)CS[C@H]12.O=S(Cl)Cl>O1CCCC1>O=C(Cc1ccccc1)N[C@@H]1C(=O)N2C(C(=O)OC(c3ccccc3)c3ccccc3)=C(CCl)CS[C@H]12
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-5eb2f821488b423cbb3ed018620cc075
CCOc1cc(N)cc2c1OCOC2.O=C(Cl)Cl.OCCF>>CCOc1cc(NC(=O)OCCF)cc2c1OCOC2
NC1=CC2=C(OCOC2)C(=C1)OCC.C(=O)(Cl)Cl.C(C)N(CC)CC.FCCO>>C(C)OC1=CC(=CC2=C1OCOC2)NC(OCCF)=O
[CH3:1][CH2:2][O:3][c:4]1[cH:5][c:6]([NH2:7])[cH:14][c:15]2[c:16]1[O:17][CH2:18][O:19][CH2:20]2.Cl[C:8](Cl)=[O:9].[OH:10][CH2:11][CH2:12][F:13]>>[CH3:1][CH2:2][O:3][c:4]1[cH:5][c:6]([NH:7][C:8](=[O:9])[O:10][CH2:11][CH2:12][F:13])[cH:14][c:15]2[c:16]1[O:17][CH2:18][O:19][CH2:20]2
CCOc1cc(N)cc2c1OCOC2.O=C(Cl)Cl.OCCF
CCOc1cc(NC(=O)OCCF)cc2c1OCOC2
null
null
C1(=CC=CC=C1)C
Protection
OtherReaction
b9a97ff2417df5b07cd245547160f318b3ee4c220885157f31c57fa8ad11f8d8
f648f3bd7738cca164e5812489428a703ee1a6f16fe0021eb651dccc8ad51d2f
c1ccc2c(c1)COCO2
Cl-[C;H0;D3;+0:1](-Cl)=[O;D1;H0:2].[C:3]-[C:4]-[OH;D1;+0:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[C:3]-[C:4]-[O;H0;D2;+0:5]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]
80.9
[{"value": 80.9, "product": "C(C)OC1=CC(=CC2=C1OCOC2)NC(OCCF)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
12
HOUR
To a solution of 6-amino-8-ethoxy-1,3-benzodioxane (1.95 g) in toluene (20 ml), a toluene solution containing phosgene (10 g) was dropwise added at 10° to 20° C. The resultant mixture was heated gradually and, after being refluxed for 30 minutes, cooled to room temperature. The solvent was removed in vacuo, whereby cru...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Acyl halide.Primary alcohol.Primary amine
Carbamic ester
null
null
c1ccc2c(c1)COCO2
HCl
C1(=CC=CC=C1)C
null
12
CCOc1cc(N)cc2c1OCOC2.O=C(Cl)Cl.OCCF>C1(=CC=CC=C1)C>CCOc1cc(NC(=O)OCCF)cc2c1OCOC2
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-323422090e9547dfb62757ce11acaab4
CCOc1cc(NC(=O)OC(C)C)cc2c1OCOC2.ClSc1ccccc1>>CCOc1cc(N(Sc2ccccc2)C(=O)OC(C)C)cc2c1OCOC2
C(C)OC1=CC(=CC2=C1OCOC2)NC(OC(C)C)=O.[H-].[Na+].C1(=CC=CC=C1)SCl>>C1(=CC=CC=C1)SN(C(OC(C)C)=O)C1=CC2=C(OCOC2)C(=C1)OCC
[CH3:1][CH2:2][O:3][c:4]1[cH:5][c:6]([NH:7][C:15](=[O:16])[O:17][CH:18]([CH3:19])[CH3:20])[cH:21][c:22]2[c:23]1[O:24][CH2:25][O:26][CH2:27]2.Cl[S:8][c:9]1[cH:10][cH:11][cH:12][cH:13][cH:14]1>>[CH3:1][CH2:2][O:3][c:4]1[cH:5][c:6]([N:7]([S:8][c:9]2[cH:10][cH:11][cH:12][cH:13][cH:14]2)[C:15](=[O:16])[O:17][CH:18]([CH3:19]...
CCOc1cc(NC(=O)OC(C)C)cc2c1OCOC2.ClSc1ccccc1
CCOc1cc(N(Sc2ccccc2)C(=O)OC(C)C)cc2c1OCOC2
null
null
CN(C=O)C
Miscellaneous
OtherReaction
904308bf2e7159b3fe00138f3899dcaffed6bbc14abc75a8cb4792c4d62a56f5
799664d421c709dc35fc986fe3317bdbac806c17bcf4a7b207ba1607f5e6b494
c1ccc(SNc2ccc3c(c2)COCO3)cc1
Cl-[S;H0;D2;+0:1]-[c:2](:[c:3]):[c:4].[C:5]-[#8:6]-[C:7](=[O;D1;H0:8])-[NH;D2;+0:9]-[c:10](:[c:11]):[c:12]>>[C:5]-[#8:6]-[C:7](=[O;D1;H0:8])-[N;H0;D3;+0:9](-[S;H0;D2;+0:1]-[c:2](:[c:3]):[c:4])-[c:10](:[c:11]):[c:12]
87.6
[{"value": 87.5, "product": "C1(=CC=CC=C1)SN(C(OC(C)C)=O)C1=CC2=C(OCOC2)C(=C1)OCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 87.6, "product": "C1(=CC=CC=C1)SN(C(OC(C)C)=O)C1=CC2=C(OCOC2)C(=C1)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
Sodium hydride (0.107 g; 60% dispersion in mineral oil) was dispersed in N,N-dimethylformamide (20 ml). To this solution was added isopropyl N-(8-ethoxy-1,3-benzodioxan-6-yl)carbamate (0.75 g) under ice-cooling. After being stirred at room temperature for 1 hour, phenylsulfenyl chloride (0.39 g) was added thereto under...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Monosulfide
Carbamic ester.Monosulfide
null
null
c1ccccc1.c1ccc2c(c1)COCO2
HCl
CN(C=O)C
null
1
CCOc1cc(NC(=O)OC(C)C)cc2c1OCOC2.ClSc1ccccc1>CN(C=O)C>CCOc1cc(N(Sc2ccccc2)C(=O)OC(C)C)cc2c1OCOC2
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-fbaca76123ad49008aae318ff22f3088
CCOC(=O)C1C(=O)N(CC)c2ccc(C3(C)OCCO3)cc21.Nc1ccc(F)cc1F>>CCN1C(=O)C(C(=O)Nc2ccc(F)cc2F)c2cc(C3(C)OCCO3)ccc21
Cl.C(Cl)Cl.C(C)N1C(C(C2=CC(=CC=C12)C1(OCCO1)C)C(=O)OCC)=O.FC1=C(N)C=CC(=C1)F>>FC1=C(C=CC(=C1)F)NC(=O)C1C(N(C2=CC=C(C=C12)C1(OCCO1)C)CC)=O
CCO[C:7]([CH:6]1[C:4](=[O:5])[N:3]([CH2:2][CH3:1])[c:29]2[c:18]1[cH:19][c:20]([C:21]1([CH3:22])[O:23][CH2:24][CH2:25][O:26]1)[cH:27][cH:28]2)=[O:8].[NH2:9][c:10]1[cH:11][cH:12][c:13]([F:14])[cH:15][c:16]1[F:17]>>[CH3:1][CH2:2][N:3]1[C:4](=[O:5])[CH:6]([C:7](=[O:8])[NH:9][c:10]2[cH:11][cH:12][c:13]([F:14])[cH:15][c:16]2...
CCOC(=O)C1C(=O)N(CC)c2ccc(C3(C)OCCO3)cc21.Nc1ccc(F)cc1F
CCN1C(=O)C(C(=O)Nc2ccc(F)cc2F)c2cc(C3(C)OCCO3)ccc21
null
null
C1=CC=CC=C1
Acylation
Aminolysis of esters
04c54ce22aa9bc0cea0de3d900446bcab51cf02bebeb606fa788a47dcd0e37ff
4335147c9ad02004b7c12428d7eac0b2e7e0e2017adc471d01c387239de8017d
O=C(Nc1ccccc1)C1C(=O)Nc2ccc(C3OCCO3)cc21
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]1-[c:4]:[c:5]-[#7:6](-[C:7])-[C:8]-1=[O;D1;H0:9].[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[C:7]-[#7:6]1-[c:5]:[c:4]-[C:3](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13])-[C:8]-1=[O;D1;H0:9]
80
[{"value": 80.0, "product": "FC1=C(C=CC(=C1)F)NC(=O)C1C(N(C2=CC=C(C=C12)C1(OCCO1)C)CC)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 1.0 g. (3.1 mmoles) of ethyl 1-ethyl-5-(2-methyl-4,5-dihydro-1,3-dioxol-2-yl)oxindole-3-carboxylate and 809 mg. (6.3 mmoles) of 2,4-difluoroaniline in 40 ml of benzene was heated to reflux through a soxhlet filled with 4A sieves for 45 minutes. The reaction mixture was cooled and poured into a mixture of 4...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccc2c(c1)CC[NH]2.C1COCO1
HO-
C1=CC=CC=C1
null
null
CCOC(=O)C1C(=O)N(CC)c2ccc(C3(C)OCCO3)cc21.Nc1ccc(F)cc1F>C1=CC=CC=C1>CCN1C(=O)C(C(=O)Nc2ccc(F)cc2F)c2cc(C3(C)OCCO3)ccc21
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-853080dc47954cab85e3613655c71d91
CCN1C(=O)C(C(=O)Nc2ccc(F)cc2F)c2cc(C3(C)OCCO3)ccc21>>CCN1C(=O)C(C(=O)Nc2ccc(F)cc2F)c2cc(C(C)=O)ccc21
FC1=C(C=CC(=C1)F)NC(=O)C1C(N(C2=CC=C(C=C12)C1(OCCO1)C)CC)=O.O1CCCC1.Cl>>FC1=C(C=CC(=C1)F)NC(=O)C1C(N(C2=CC=C(C=C12)C(C)=O)CC)=O
C1C[O:23][C:21]([c:20]2[cH:19][c:18]3[c:26]([cH:25][cH:24]2)[N:3]([CH2:2][CH3:1])[C:4](=[O:5])[CH:6]3[C:7](=[O:8])[NH:9][c:10]2[cH:11][cH:12][c:13]([F:14])[cH:15][c:16]2[F:17])([CH3:22])O1>>[CH3:1][CH2:2][N:3]1[C:4](=[O:5])[CH:6]([C:7](=[O:8])[NH:9][c:10]2[cH:11][cH:12][c:13]([F:14])[cH:15][c:16]2[F:17])[c:18]2[cH:19][...
CCN1C(=O)C(C(=O)Nc2ccc(F)cc2F)c2cc(C3(C)OCCO3)ccc21
CCN1C(=O)C(C(=O)Nc2ccc(F)cc2F)c2cc(C(C)=O)ccc21
null
null
O
Miscellaneous
Ketal hydrolysis to ketone
bc99a45944d6d67c8bd263755d04463b42623d20ce36570ebfd14e405f44ca50
547697208447432e865290cf95eed8e4fcddc12f59856b7ddbf24dc1accb1210
O=C(Nc1ccccc1)C1C(=O)Nc2ccccc21
[C;D1;H3:1]-[C;H0;D4;+0:2]1(-[c:3](:[c:4]):[c:5])-O-C-C-[O;H0;D2;+0:6]-1>>[C;D1;H3:1]-[C;H0;D3;+0:2](=[O;H0;D1;+0:6])-[c:3](:[c:4]):[c:5]
73
[{"value": 73.0, "product": "FC1=C(C=CC(=C1)F)NC(=O)C1C(N(C2=CC=C(C=C12)C(C)=O)CC)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
N-(2,4-Difluorophenyl)-1-ethyl-5-(2-methyl-4,5-dihydro-1,3-dioxol-2-yl)oxindol-3-carboxamide (636 mg., 1.58 mmoles) was dissolved in 15 ml. of tetrahydrofuran to which was added 10 ml. of 1N hydrochloric acid. The solution was stirred for one hour followed by the addition of an equal volume of water. The resulting prec...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether
Ketone
C1COCO1
null
c1ccccc1.c1ccc2c(c1)CC[NH]2
HO-
O
null
1
CCN1C(=O)C(C(=O)Nc2ccc(F)cc2F)c2cc(C3(C)OCCO3)ccc21>O>CCN1C(=O)C(C(=O)Nc2ccc(F)cc2F)c2cc(C(C)=O)ccc21
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-de8eb938f854499db8dc033cab51fe90
CCN1C(=O)Cc2ccccc21>>CCN1C(=O)Cc2cc(C=O)ccc21
COC(Cl)Cl.C(C)N1C(CC2=CC=CC=C12)=O.COC(Cl)Cl>>C(C)N1C(CC2=CC(=CC=C12)C=O)=O
[CH3:1][CH2:2][N:3]1[C:4](=[O:5])[CH2:6][c:7]2[cH:8][cH:9][cH:12][cH:13][c:14]21>>[CH3:1][CH2:2][N:3]1[C:4](=[O:5])[CH2:6][c:7]2[cH:8][c:9]([CH:10]=[O:11])[cH:12][cH:13][c:14]21
CCN1C(=O)Cc2ccccc21
CCN1C(=O)Cc2cc(C=O)ccc21
null
[Ti](Cl)(Cl)(Cl)Cl.[Ti](Cl)(Cl)(Cl)Cl
C(Cl)Cl
Miscellaneous
OtherReaction
7411dfc8672888ceb211fc5e1d3019bf18f4b5648ebb82adb2b5243009e4359d
3cccf922e74135722ee21a46ad7578302a8603e1f71d6f2113cd42de4ba0cf73
O=C1Cc2ccccc2N1
[c:1]:[c:2]:[cH;D2;+0:3]:[c:4]:[c:5]>>[O;D1;H0:6]=[C:7]-[c;H0;D3;+0:3](:[c:2]:[c:1]):[c:4]:[c:5]
76
[{"value": 76.0, "product": "C(C)N1C(CC2=CC(=CC=C12)C=O)=O", "details": "PERCENTYIELD", "is_desired": false}]
25
CELSIUS
10.5
DAY
To a solution of 32.2 g. (0.2 mole) of 1-ethyloxindole in 200 ml. of methylene chloride was added 44 ml. (0.4 mole) of titanium tetrachloride followed by 22.6 ml. (0.25 mole) of dichloromethyl methyl ether. The reaction was stirred for 10.5 days at 25° C. followed by the addition of additional titanium tetrachloride an...
10.6084/m9.figshare.5104873.v1
null
null
Aldehyde
c1ccc2c(c1)CC[NH]2
c1ccc2c(c1)CC[NH]2
c1ccc2c(c1)CC[NH]2
Other
[Ti](Cl)(Cl)(Cl)Cl.[Ti](Cl)(Cl)(Cl)Cl.C(Cl)Cl
25
252
CCN1C(=O)Cc2ccccc21>[Ti](Cl)(Cl)(Cl)Cl.[Ti](Cl)(Cl)(Cl)Cl.C(Cl)Cl>CCN1C(=O)Cc2cc(C=O)ccc21
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-13d693696b6c40afae66096a9a28bbb9
CCN1C(=O)Cc2cc(CCC(=O)OC)ccc21>>CCN1C(=O)Cc2cc(CCC(=O)O)ccc21
C(C)N1C(CC2=CC(=CC=C12)CCC(=O)OC)=O.[OH-].[Na+].Cl>>C(C)N1C(CC2=CC(=CC=C12)CCC(=O)O)=O
C[O:14][C:12]([CH2:11][CH2:10][c:9]1[cH:8][c:7]2[c:17]([cH:16][cH:15]1)[N:3]([CH2:2][CH3:1])[C:4](=[O:5])[CH2:6]2)=[O:13]>>[CH3:1][CH2:2][N:3]1[C:4](=[O:5])[CH2:6][c:7]2[cH:8][c:9]([CH2:10][CH2:11][C:12](=[O:13])[OH:14])[cH:15][cH:16][c:17]21
CCN1C(=O)Cc2cc(CCC(=O)OC)ccc21
CCN1C(=O)Cc2cc(CCC(=O)O)ccc21
null
null
CO
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C1Cc2ccccc2N1
C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
93
[{"value": 93.0, "product": "C(C)N1C(CC2=CC(=CC=C12)CCC(=O)O)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a solution of 12.9 g. (52.2 mmoles) of 1-ethyl-5-(2-carbomethoxyethyl)oxindole in 53 ml. of methanol was added 112.5 ml. of 1N sodium hydroxide solution. After stirring for 1 hour the reaction mixture was acidified by the addition of 165 ml. of 1N hydrochloric acid. The precipitated product was filtered and dried, 1...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccc2c(c1)CC[NH]2
Other
CO
null
1
CCN1C(=O)Cc2cc(CCC(=O)OC)ccc21>CO>CCN1C(=O)Cc2cc(CCC(=O)O)ccc21
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-1e2ecc46940240de9aedcef37e969379
CCCN1C(=O)Cc2cc3c(cc21)C(=O)CC3>>CCN1C(=O)Cc2cc3c(cc21)C(=O)CC3
CN1C(CC2=CC3=C(C=C12)C(CC3)=O)=O.C1(=CC=CC=C1)N1C(CC2=CC3=C(C=C12)C(CC3)=O)=O.C(CC)N1C(CC2=CC3=C(C=C12)C(CC3)=O)=O.C(C)(C)N1C(CC2=CC3=C(C=C12)C(CC3)=O)=O>>C(C)N1C(CC2=CC3=C(C=C12)C(CC3)=O)=O
C[CH2:1][CH2:2][N:3]1[C:4](=[O:5])[CH2:6][c:7]2[cH:8][c:9]3[c:10]([cH:11][c:12]21)[C:13](=[O:14])[CH2:15][CH2:16]3>>[CH3:1][CH2:2][N:3]1[C:4](=[O:5])[CH2:6][c:7]2[cH:8][c:9]3[c:10]([cH:11][c:12]21)[C:13](=[O:14])[CH2:15][CH2:16]3
CCCN1C(=O)Cc2cc3c(cc21)C(=O)CC3
CCN1C(=O)Cc2cc3c(cc21)C(=O)CC3
null
null
null
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
O=C1Cc2cc3c(cc2N1)C(=O)CC3
C-[CH2;D2;+0:1]-[C:2]-[#7:3]-[C:4]=[O;D1;H0:5]>>[CH3;D1;+0:1]-[C:2]-[#7:3]-[C:4]=[O;D1;H0:5]
null
[]
null
null
null
null
Starting with the appropriate 1-substituted-5-hydroxyoxindole and following the procedure of Preparation A, 1-methyl-2,7-dioxo-2,3,5,6-tetrahydro-7H-cyclopenta[f]indole, 1-phenyl-2,7-dioxo-2,3,5,6-tetrahydro-7H-cyclopenta[f]indole, 1-n-propyl-2,7-dioxo-2,3,5,6-tetrahydro-7H-cyclopenta[f]indole and 1-i-propyl-2,7-dioxo-...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
c1c2c(cc3c1CC[NH]3)CCC2
Other
null
null
null
CCCN1C(=O)Cc2cc3c(cc21)C(=O)CC3>>CCN1C(=O)Cc2cc3c(cc21)C(=O)CC3
ord_dataset-c34472859da14a81bfe0f74e60f15c43
ord-e92da1eef89c454781325f5bee029024
CCN1C(=O)Cc2cc(O)ccc21.O=C(Cl)CCl>>CCN1C(=O)Cc2cc(OC(=O)CCl)ccc21
C(C)N1C(CC2=CC(=CC=C12)O)=O.ClCC(=O)Cl.N1=CC=CC=C1>>C(C)N1C(CC2=CC(=CC=C12)OC(CCl)=O)=O
[CH3:1][CH2:2][N:3]1[C:4](=[O:5])[CH2:6][c:7]2[cH:8][c:9]([OH:10])[cH:15][cH:16][c:17]21.Cl[C:11](=[O:12])[CH2:13][Cl:14]>>[CH3:1][CH2:2][N:3]1[C:4](=[O:5])[CH2:6][c:7]2[cH:8][c:9]([O:10][C:11](=[O:12])[CH2:13][Cl:14])[cH:15][cH:16][c:17]21
CCN1C(=O)Cc2cc(O)ccc21.O=C(Cl)CCl
CCN1C(=O)Cc2cc(OC(=O)CCl)ccc21
null
null
ClCCl
Acylation
Schotten-Baumann to ester
1cda078f55e64d9385e544d1067595d5e7672bbd1eff542e7a341817a2d8c4d5
6439fc27f97ee9ed7c11ef9b5032d9493d05f28a7bbb50d256a2d54d035fbfb2
O=C1Cc2ccccc2N1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[Cl;D1;H0:4].[OH;D1;+0:5]-[c:6](:[c:7]):[c:8]>>[Cl;D1;H0:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[O;H0;D2;+0:5]-[c:6](:[c:7]):[c:8]
null
[]
null
null
15
MINUTE
To a slurry of 100 g. (0.565 mole) of 1-ethyl-5-hydroxyoxindole in 91.3 ml. (1.13 moles) of pyridine and 565 ml. of dichloromethane at 0° C. was added dropwise a solution of 89.3 ml. (1.13 moles) of chloroacetyl chloride in 100 ml. of dichloromethane. The reaction mixture was allowed to stir for 15 minutes, and was the...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Aromatic alcohol
Ester
null
null
c1ccc2c(c1)CC[NH]2
HCl
ClCCl
null
0.25
CCN1C(=O)Cc2cc(O)ccc21.O=C(Cl)CCl>ClCCl>CCN1C(=O)Cc2cc(OC(=O)CCl)ccc21