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414 values
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36
36
reaction_smiles
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4
873
rxn_insight_reaction
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19
1.07k
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14
3.37k
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large_stringlengths
1
581
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1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
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large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
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large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c8a6c66353b048e0bd9410b9648b22b8
CN(C)CCCn1ncc2ccc([N+](=O)[O-])cc21>>CN(C)CCCn1ncc2ccc(N)cc21
CN(CCCN1N=CC2=CC=C(C=C12)[N+](=O)[O-])C.[Cl-].[NH4+]>>CN(CCCN1N=CC2=CC=C(C=C12)N)C
O=[N+:14]([O-])[c:13]1[cH:12][cH:11][c:10]2[cH:9][n:8][n:7]([CH2:6][CH2:5][CH2:4][N:2]([CH3:1])[CH3:3])[c:16]2[cH:15]1>>[CH3:1][N:2]([CH3:3])[CH2:4][CH2:5][CH2:6][n:7]1[n:8][cH:9][c:10]2[cH:11][cH:12][c:13]([NH2:14])[cH:15][c:16]12
CN(C)CCCn1ncc2ccc([N+](=O)[O-])cc21
CN(C)CCCn1ncc2ccc(N)cc21
null
[Fe]
C(C)O.O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc2[nH]ncc2c1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]:[c:5]:[#7;a:6]>>[#7;a:6]:[c:5]:[c:4]:[c:2](-[NH2;D1;+0:1]):[c:3]
null
[]
null
null
15
MINUTE
A mixture of dimethyl-{3-(6-nitro-indazol-1-yl)-propyl}-amine (0.400 g, 1.61 mmol), iron powder (0.897 g, 16.1 mmol), and ammonium chloride (0.0430 mg, 0.811 mmol) in a 4:1 solution of ethanol/H2O was heated to reflux for 3 hours, cooled to room temperature and concentrated under reduced pressure. The residue was taken...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccc2cn[nH]c2c1
Other
[Fe].C(C)O.O
null
0.25
CN(C)CCCn1ncc2ccc([N+](=O)[O-])cc21>[Fe].C(C)O.O>CN(C)CCCn1ncc2ccc(N)cc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-931258ae9c17455eb502585125c483a9
Cl.O=[N+]([O-])c1cccc2[nH]ncc12>>O=[N+]([O-])c1cccc2[nH]nc(Cl)c12
Cl.[N+](=O)([O-])C1=C2C=NNC2=CC=C1.[OH-].[Na+].[O-]Cl.[Na+]>>ClC1=NNC2=CC=CC(=C12)[N+](=O)[O-]
[ClH:12].[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][cH:7][c:8]2[nH:9][n:10][cH:11][c:13]12>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][cH:7][c:8]2[nH:9][n:10][c:11]([Cl:12])[c:13]12
Cl.O=[N+]([O-])c1cccc2[nH]ncc12
O=[N+]([O-])c1cccc2[nH]nc(Cl)c12
null
null
O
Functional Group Addition
Chlorination
d7565c0d49fd3424f26a8edf0928ad120b0a003a57177c1e3e1e6ba6fde6a68c
0a2f22058f27970cef4a98a778644dbe9c44e91f66c74cd24db321993177608a
c1ccc2[nH]ncc2c1
[ClH;D0;+0:1].[c:2]:[c:3]1:[cH;D2;+0:4]:[#7;a:5]:[#7;a:6]:[c:7]:1:[c:8]>>[Cl;H0;D1;+0:1]-[c;H0;D3;+0:4]1:[#7;a:5]:[#7;a:6]:[c:7](:[c:8]):[c:3]:1:[c:2]
null
[]
0
CELSIUS
5
HOUR
To a mixture of NaOH (0.500 g, 12.5 mmol) in H2O (15.0 mL) was added 4-nitroindazole (0.500 g, 3.07 mmol) after which it was heated until a red solution formed. The solution was immediately placed in an ice-water bath for 15 minutes before NaClO (6.00 mL, 5.25%, 4.50 mmol) was added. The mixture was stirred at 0° C. fo...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2[nH]ncc2c1
c1ccc2[nH]ncc2c1
c1ccc2[nH]ncc2c1
null
O
0
5
Cl.O=[N+]([O-])c1cccc2[nH]ncc12>O>O=[N+]([O-])c1cccc2[nH]nc(Cl)c12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-8f1ce3ca17d440acba30939cbb5f2814
ClCCN1CCCC1.O=[N+]([O-])c1cccc2[nH]nc(Cl)c12>>O=[N+]([O-])c1cccc2c1c(Cl)nn2CCN1CCCC1
ClC1=NNC2=CC=CC(=C12)[N+](=O)[O-].C([O-])([O-])=O.[K+].[K+].Cl.ClCCN1CCCC1>>ClC1=NN(C2=CC=CC(=C12)[N+](=O)[O-])CCN1CCCC1
Cl[CH2:14][CH2:15][N:16]1[CH2:17][CH2:18][CH2:19][CH2:20]1.[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][cH:7][c:8]2[c:9]1[c:10]([Cl:11])[n:12][nH:13]2>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][cH:7][c:8]2[c:9]1[c:10]([Cl:11])[n:12][n:13]2[CH2:14][CH2:15][N:16]1[CH2:17][CH2:18][CH2:19][CH2:20]1
ClCCN1CCCC1.O=[N+]([O-])c1cccc2[nH]nc(Cl)c12
O=[N+]([O-])c1cccc2c1c(Cl)nn2CCN1CCCC1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
37f45c65843eb1934d1248942acee56370679d83d9e5e49713f458cd256ddf5b
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ccc2c(c1)cnn2CCN1CCCC1
Cl-[CH2;D2;+0:1]-[C:2]-[#7:3].[c:4]:[c:5]1:[c:6]:[c:7]:[#7;a:8]:[nH;D2;+0:9]:1>>[#7:3]-[C:2]-[CH2;D2;+0:1]-[n;H0;D3;+0:9]1:[#7;a:8]:[c:7]:[c:6]:[c:5]:1:[c:4]
null
[]
50
CELSIUS
null
null
A mixture of 3-chloro-4-nitro-1H-indazole (0.550 g, 2.79 mmol) was treated with potassium carbonate (1.20 g 8.70 mmol) in DMF (10 mL) for 30 minutes, after which 1-(2-chloro-ethyl)-pyrrolidine hydrochloride (0.710 g, 4.20 mmol) was added. The mixture was heated to 50° C. for 6 hours, cooled to room temperature and filt...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ccc2n[nH]cc2c1
c1cccc2n[nH]cc12
c1cccc2n[nH]cc12.C1CC[NH]C1
HCl
CN(C)C=O
50
null
ClCCN1CCCC1.O=[N+]([O-])c1cccc2[nH]nc(Cl)c12>CN(C)C=O>O=[N+]([O-])c1cccc2c1c(Cl)nn2CCN1CCCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f97ad5d0f3d14ad3bcc2c20530fae0e5
O=[N+]([O-])c1cccc2c1c(Cl)nn2CCN1CCCC1>>Nc1cccc2c1c(Cl)nn2CCN1CCCC1
ClC1=NN(C2=CC=CC(=C12)[N+](=O)[O-])CCN1CCCC1.[Cl-].[NH4+]>>ClC1=NN(C2=CC=CC(=C12)N)CCN1CCCC1
O=[N+:1]([O-])[c:2]1[cH:3][cH:4][cH:5][c:6]2[c:7]1[c:8]([Cl:9])[n:10][n:11]2[CH2:12][CH2:13][N:14]1[CH2:15][CH2:16][CH2:17][CH2:18]1>>[NH2:1][c:2]1[cH:3][cH:4][cH:5][c:6]2[c:7]1[c:8]([Cl:9])[n:10][n:11]2[CH2:12][CH2:13][N:14]1[CH2:15][CH2:16][CH2:17][CH2:18]1
O=[N+]([O-])c1cccc2c1c(Cl)nn2CCN1CCCC1
Nc1cccc2c1c(Cl)nn2CCN1CCCC1
null
[Fe]
C(C)O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc2c(c1)cnn2CCN1CCCC1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]1:[c:5]:[#7;a:6]:[#7;a:7]:[c:8]:1>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]1:[c:5]:[#7;a:6]:[#7;a:7]:[c:8]:1
84
[{"value": 84.0, "product": "ClC1=NN(C2=CC=CC(=C12)N)CCN1CCCC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 80.9, "product": "ClC1=NN(C2=CC=CC(=C12)N)CCN1CCCC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
A mixture of 3-Chloro-4-nitro-1-(2-pyrrolidin-1-yl-ethyl)-1H-indazole (0.40 g, 1.4 mmol), iron powder (0.76 g, 14 mmol), and ammonium chloride (37 mg, 0.68 mmol) in 80% Ethanol was heated to reflux for 3 hours, cooled to room temperature and concentrated under reduced pressure. The residue was stirred in triethylamine/...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1cccc2n[nH]cc12.C1CC[NH]C1
Other
[Fe].C(C)O
null
0.25
O=[N+]([O-])c1cccc2c1c(Cl)nn2CCN1CCCC1>[Fe].C(C)O>Nc1cccc2c1c(Cl)nn2CCN1CCCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4e118547db8643f1873744afbd99b347
Nc1cccc2c1c(Cl)nn2CCN1CCCC1.O=C(O)Cc1ccc(OCc2ccccc2)cc1>>O=C(Cc1ccc(OCc2ccccc2)cc1)Nc1cccc2c1c(Cl)nn2CCN1CCCC1
ClC1=NN(C2=CC=CC(=C12)N)CCN1CCCC1.C(C1=CC=CC=C1)OC1=CC=C(C=C1)CC(=O)O.Cl.C(C)N=C=NC(CC)(C)C.ON1N=NC2=C1C=CC=C2.CN1CCOCC1>>C(C1=CC=CC=C1)OC1=CC=C(C=C1)CC(=O)NC1=C2C(=NN(C2=CC=C1)CCN1CCCC1)Cl
[NH2:18][c:19]1[cH:20][cH:21][cH:22][c:23]2[c:24]1[c:25]([Cl:26])[n:27][n:28]2[CH2:29][CH2:30][N:31]1[CH2:32][CH2:33][CH2:34][CH2:35]1.O[C:2](=[O:1])[CH2:3][c:4]1[cH:5][cH:6][c:7]([O:8][CH2:9][c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[cH:16][cH:17]1>>[O:1]=[C:2]([CH2:3][c:4]1[cH:5][cH:6][c:7]([O:8][CH2:9][c:10]2[cH:1...
Nc1cccc2c1c(Cl)nn2CCN1CCCC1.O=C(O)Cc1ccc(OCc2ccccc2)cc1
O=C(Cc1ccc(OCc2ccccc2)cc1)Nc1cccc2c1c(Cl)nn2CCN1CCCC1
null
null
CN(C)C=O
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Cc1ccc(OCc2ccccc2)cc1)Nc1cccc2c1cnn2CCN1CCCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[c:4].[NH2;D1;+0:5]-[c:6](:[c:7]):[c:8]1:[c:9]:[#7;a:10]:[#7;a:11]:[c:12]:1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[C:3]-[c:4])-[NH;D2;+0:5]-[c:6](:[c:7]):[c:8]1:[c:9]:[#7;a:10]:[#7;a:11]:[c:12]:1
null
[]
null
null
6
HOUR
A mixture of 3-chloro-1-(2-pyrrolidin-1-yl-ethyl)-1H-indazol-4-ylamine (300 mg, 1.14 mmol), (4-benzyloxy-phenyl)-acetic acid (302 mg, 1.25 mmol), ethyldimethylpropylcarbodiimide hydrochloride (261 mg g, 1.37 mmol), N-hydroxybenzotriazole (184 mg, 1.37 mmol), N-methyl morpholine (290 mg, 2.72 mmol) in 5 mL of DMF was st...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccccc1.c1cccc2n[nH]cc12.C1CC[NH]C1
HO-
CN(C)C=O
null
6
Nc1cccc2c1c(Cl)nn2CCN1CCCC1.O=C(O)Cc1ccc(OCc2ccccc2)cc1>CN(C)C=O>O=C(Cc1ccc(OCc2ccccc2)cc1)Nc1cccc2c1c(Cl)nn2CCN1CCCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c6bb2a64285e402fb31d762dc9f96674
O=C(Cc1ccc(OCc2ccccc2)cc1)Nc1cccc2c1cnn2CCN1CCCC1.[Br-]>>O=C(Cc1ccc(OCc2ccccc2)cc1)Nc1cccc2c1c(Br)nn2CCN1CCCC1
Cl.C(C1=CC=CC=C1)OC1=CC=C(C=C1)CC(=O)NC1=C2C=NN(C2=CC=C1)CCN1CCCC1.[OH-].[Na+].[Br-].[Br-].[Br-].[NH+]1=CC=CC=C1.[NH+]1=CC=CC=C1.[NH+]1=CC=CC=C1>>C(C1=CC=CC=C1)OC1=CC=C(C=C1)CC(=O)NC1=C2C(=NN(C2=CC=C1)CCN1CCCC1)Br
[O:1]=[C:2]([CH2:3][c:4]1[cH:5][cH:6][c:7]([O:8][CH2:9][c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[cH:16][cH:17]1)[NH:18][c:19]1[cH:20][cH:21][cH:22][c:23]2[c:24]1[cH:25][n:27][n:28]2[CH2:29][CH2:30][N:31]1[CH2:32][CH2:33][CH2:34][CH2:35]1.[Br-:26]>>[O:1]=[C:2]([CH2:3][c:4]1[cH:5][cH:6][c:7]([O:8][CH2:9][c:10]2[cH:11]...
O=C(Cc1ccc(OCc2ccccc2)cc1)Nc1cccc2c1cnn2CCN1CCCC1.[Br-]
O=C(Cc1ccc(OCc2ccccc2)cc1)Nc1cccc2c1c(Br)nn2CCN1CCCC1
null
null
O.CO
Functional Group Interconversion
Bromination
25157f9d3af4ae241d48d9986ef2032af184156718cdc4bc554e8a3105505db7
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
O=C(Cc1ccc(OCc2ccccc2)cc1)Nc1cccc2c1cnn2CCN1CCCC1
[Br-;H0;D0:1].[C:2]-[#7;a:3]1:[#7;a:4]:[cH;D2;+0:5]:[c:6](:[c:7]):[c:8]:1:[c:9]>>[Br;H0;D1;+0:1]-[c;H0;D3;+0:5]1:[#7;a:4]:[#7;a:3](-[C:2]):[c:8](:[c:9]):[c:6]:1:[c:7]
null
[]
0
CELSIUS
5
HOUR
A mixture of 2-[4-(benzyloxy)phenyl]-N-[1-(2-pyrrolidin-1-ylethyl)-1H-indazol-4-yl]acetamide (Example 3, 0.200 g, 0.440 mmol) and NaOH (0.400 g, 10.0 mmol) in H2O (6 mL) was added in methanol (6 mL) was placed in an ice-water bath for 15 minutes before pyridinium tribromide (0.470 g, 1.47 mmol) in MeOH (1.5 mL) was add...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1cccc2n[nH]cc12
c1cccc2n[nH]cc12
c1ccccc1.c1ccccc1.c1cccc2n[nH]cc12.C1CC[NH]C1
null
O.CO
0
5
O=C(Cc1ccc(OCc2ccccc2)cc1)Nc1cccc2c1cnn2CCN1CCCC1.[Br-]>O.CO>O=C(Cc1ccc(OCc2ccccc2)cc1)Nc1cccc2c1c(Br)nn2CCN1CCCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-3186eb8c24f146f1a18c81ee9a18bf8e
Cl.O=[N+]([O-])c1ccc2[nH]ncc2c1>>O=[N+]([O-])c1ccc2[nH]nc(Cl)c2c1
Cl.[N+](=O)([O-])C=1C=C2C=NNC2=CC1.[OH-].[Na+].[O-]Cl.[Na+]>>ClC1=NNC2=CC=C(C=C12)[N+](=O)[O-]
[ClH:11].[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]2[nH:8][n:9][cH:10][c:12]2[cH:13]1>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]2[nH:8][n:9][c:10]([Cl:11])[c:12]2[cH:13]1
Cl.O=[N+]([O-])c1ccc2[nH]ncc2c1
O=[N+]([O-])c1ccc2[nH]nc(Cl)c2c1
null
null
O
Functional Group Addition
Chlorination
d7565c0d49fd3424f26a8edf0928ad120b0a003a57177c1e3e1e6ba6fde6a68c
0a2f22058f27970cef4a98a778644dbe9c44e91f66c74cd24db321993177608a
c1ccc2[nH]ncc2c1
[ClH;D0;+0:1].[c:2]:[c:3]1:[cH;D2;+0:4]:[#7;a:5]:[#7;a:6]:[c:7]:1:[c:8]>>[Cl;H0;D1;+0:1]-[c;H0;D3;+0:4]1:[#7;a:5]:[#7;a:6]:[c:7](:[c:8]):[c:3]:1:[c:2]
92
[{"value": 92.0, "product": "ClC1=NNC2=CC=C(C=C12)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 90.7, "product": "ClC1=NNC2=CC=C(C=C12)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
5
HOUR
A mixture of NaOH (5.00 g, 125 mmol) in H2O (150 mL) was added 5-nitroindazole (5.00 g, 30.7 mmol), and the mixture was heated until a red solution formed. The mixture was cooled in an ice-water bath for 15 minutes, NaClO (60.0 mL, 5.25%, 45.0 mmol) was added and the mixture stirred at 0° C. for 5 hour after which the ...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2[nH]ncc2c1
c1ccc2[nH]ncc2c1
c1ccc2[nH]ncc2c1
null
O
0
5
Cl.O=[N+]([O-])c1ccc2[nH]ncc2c1>O>O=[N+]([O-])c1ccc2[nH]nc(Cl)c2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a37e2a2096fd472dbd96dba73ca65231
ClCCN1CCCC1.O=[N+]([O-])c1ccc2[nH]nc(Cl)c2c1>>O=[N+]([O-])c1ccc2c(c1)c(Cl)nn2CCN1CCCC1
ClC1=NNC2=CC=C(C=C12)[N+](=O)[O-].C([O-])([O-])=O.[K+].[K+].ClCCN1CCCC1>>ClC1=NN(C2=CC=C(C=C12)[N+](=O)[O-])CCN1CCCC1
Cl[CH2:14][CH2:15][N:16]1[CH2:17][CH2:18][CH2:19][CH2:20]1.[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]2[c:8]([cH:9]1)[c:10]([Cl:11])[n:12][nH:13]2>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]2[c:8]([cH:9]1)[c:10]([Cl:11])[n:12][n:13]2[CH2:14][CH2:15][N:16]1[CH2:17][CH2:18][CH2:19][CH2:20]1
ClCCN1CCCC1.O=[N+]([O-])c1ccc2[nH]nc(Cl)c2c1
O=[N+]([O-])c1ccc2c(c1)c(Cl)nn2CCN1CCCC1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
1c9bfadcc8b17ce33571db0aba6fe4d2adf28d49d529bcf12a641e342e01b0dc
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ccc2c(c1)cnn2CCN1CCCC1
Cl-[CH2;D2;+0:1]-[C:2]-[#7:3].[c:4]:[c:5]1:[c:6]:[c:7]:[#7;a:8]:[nH;D2;+0:9]:1>>[#7:3]-[C:2]-[CH2;D2;+0:1]-[n;H0;D3;+0:9]1:[#7;a:8]:[c:7]:[c:6]:[c:5]:1:[c:4]
null
[]
50
CELSIUS
null
null
A mixture of 3-chloro-5-nitro-1H-indazole (1.5 g, 7.6 mmol) was treated with potassium carbonate (3.1 g, 23 mmol) in DMF (20 mL) for 30 minutes, after which 1-(2-chloro-ethyl)-pyrrolidine (1.9 g, 11 mmol) was added. The mixture was heated to 50° C. for 6 hours, cooled to room temperature, filtered through a plug of sil...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ccc2n[nH]cc2c1
c1ccc2n[nH]cc2c1
c1ccc2n[nH]cc2c1.C1CC[NH]C1
HCl
CN(C)C=O
50
null
ClCCN1CCCC1.O=[N+]([O-])c1ccc2[nH]nc(Cl)c2c1>CN(C)C=O>O=[N+]([O-])c1ccc2c(c1)c(Cl)nn2CCN1CCCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c1aafaf9b8134916a2f3fa6a6260862d
O=[N+]([O-])c1ccc2c(c1)c(Cl)nn2CCN1CCCC1>>Nc1ccc2c(c1)c(Cl)nn2CCN1CCCC1
ClC1=NN(C2=CC=C(C=C12)[N+](=O)[O-])CCN1CCCC1.[Cl-].[NH4+]>>ClC1=NN(C2=CC=C(C=C12)N)CCN1CCCC1
O=[N+:1]([O-])[c:2]1[cH:3][cH:4][c:5]2[c:6]([cH:7]1)[c:8]([Cl:9])[n:10][n:11]2[CH2:12][CH2:13][N:14]1[CH2:15][CH2:16][CH2:17][CH2:18]1>>[NH2:1][c:2]1[cH:3][cH:4][c:5]2[c:6]([cH:7]1)[c:8]([Cl:9])[n:10][n:11]2[CH2:12][CH2:13][N:14]1[CH2:15][CH2:16][CH2:17][CH2:18]1
O=[N+]([O-])c1ccc2c(c1)c(Cl)nn2CCN1CCCC1
Nc1ccc2c(c1)c(Cl)nn2CCN1CCCC1
null
[Fe]
C(C)O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc2c(c1)cnn2CCN1CCCC1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
84
[{"value": 84.0, "product": "ClC1=NN(C2=CC=C(C=C12)N)CCN1CCCC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 80.9, "product": "ClC1=NN(C2=CC=C(C=C12)N)CCN1CCCC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
A mixture of 3-Chloro-5-nitro-1-(2-pyrrolidin-1-yl-ethyl)-1H-indazole (0.40 g, 1.4 mmol), iron powder (0.76 g, 14 mmol), and ammonium chloride (37 mg, 0.68 mmol) in 80% ethanol was heated to reflux for 3 hours, cooled to room temperature and concentrated under reduced pressure. The residue was stirred in triethylamine/...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccc2n[nH]cc2c1.C1CC[NH]C1
Other
[Fe].C(C)O
null
0.25
O=[N+]([O-])c1ccc2c(c1)c(Cl)nn2CCN1CCCC1>[Fe].C(C)O>Nc1ccc2c(c1)c(Cl)nn2CCN1CCCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-cc15a859aa5645abafbaf42d9c833fd3
O=[N+]([O-])c1ccc2[nH]ncc2c1.[Br-]>>O=[N+]([O-])c1ccc2[nH]nc(Br)c2c1
Cl.[N+](=O)([O-])C=1C=C2C=NNC2=CC1.[OH-].[Na+].[Br-].[Br-].[Br-].[NH+]1=CC=CC=C1.[NH+]1=CC=CC=C1.[NH+]1=CC=CC=C1>>BrC1=NNC2=CC=C(C=C12)[N+](=O)[O-]
[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]2[nH:8][n:9][cH:10][c:12]2[cH:13]1.[Br-:11]>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]2[nH:8][n:9][c:10]([Br:11])[c:12]2[cH:13]1
O=[N+]([O-])c1ccc2[nH]ncc2c1.[Br-]
O=[N+]([O-])c1ccc2[nH]nc(Br)c2c1
null
null
O.CO
Functional Group Interconversion
Bromination
c227dfbda497353373bac89bc247ec5b3f58de92ee9133ce1c0d94d6b7643f7c
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1ccc2[nH]ncc2c1
[Br-;H0;D0:1].[c:2]:[c:3]1:[cH;D2;+0:4]:[#7;a:5]:[#7;a:6]:[c:7]:1:[c:8]>>[Br;H0;D1;+0:1]-[c;H0;D3;+0:4]1:[#7;a:5]:[#7;a:6]:[c:7](:[c:8]):[c:3]:1:[c:2]
55.1
[{"value": 55.0, "product": "BrC1=NNC2=CC=C(C=C12)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 55.1, "product": "BrC1=NNC2=CC=C(C=C12)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
15
MINUTE
A mixture of NaOH (2.0 g) in H2O (60 mL) was added 5-nitroindazole (2.0 g, 12 mmol), and the mixture was heated until a red solution formed. The mixture was placed in an ice-water bath for 15 minutes after which pyridinium tribromide (4.7 g, 15 mmol) in methanol (15 mL) was added. The mixture was stirred at 0° C. for 5...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2[nH]ncc2c1
c1ccc2[nH]ncc2c1
c1ccc2[nH]ncc2c1
null
O.CO
0
0.25
O=[N+]([O-])c1ccc2[nH]ncc2c1.[Br-]>O.CO>O=[N+]([O-])c1ccc2[nH]nc(Br)c2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f5e25737fd3846fd89334f3669445254
ClCCN1CCCC1.O=[N+]([O-])c1ccc2[nH]nc(Br)c2c1>>O=[N+]([O-])c1ccc2c(c1)c(Br)nn2CCN1CCCC1
BrC1=NNC2=CC=C(C=C12)[N+](=O)[O-].C([O-])([O-])=O.[K+].[K+].ClCCN1CCCC1>>BrC1=NN(C2=CC=C(C=C12)[N+](=O)[O-])CCN1CCCC1
Cl[CH2:14][CH2:15][N:16]1[CH2:17][CH2:18][CH2:19][CH2:20]1.[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]2[c:8]([cH:9]1)[c:10]([Br:11])[n:12][nH:13]2>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]2[c:8]([cH:9]1)[c:10]([Br:11])[n:12][n:13]2[CH2:14][CH2:15][N:16]1[CH2:17][CH2:18][CH2:19][CH2:20]1
ClCCN1CCCC1.O=[N+]([O-])c1ccc2[nH]nc(Br)c2c1
O=[N+]([O-])c1ccc2c(c1)c(Br)nn2CCN1CCCC1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
1c9bfadcc8b17ce33571db0aba6fe4d2adf28d49d529bcf12a641e342e01b0dc
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ccc2c(c1)cnn2CCN1CCCC1
Cl-[CH2;D2;+0:1]-[C:2]-[#7:3].[c:4]:[c:5]1:[c:6]:[c:7]:[#7;a:8]:[nH;D2;+0:9]:1>>[#7:3]-[C:2]-[CH2;D2;+0:1]-[n;H0;D3;+0:9]1:[#7;a:8]:[c:7]:[c:6]:[c:5]:1:[c:4]
133.4
[{"value": 76.0, "product": "BrC1=NN(C2=CC=C(C=C12)[N+](=O)[O-])CCN1CCCC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 133.4, "product": "BrC1=NN(C2=CC=C(C=C12)[N+](=O)[O-])CCN1CCCC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
50
CELSIUS
null
null
A mixture of 3-bromo-5-nitro-1H-indazole (1.8 g, 7.6 mmol) and potassium carbonate (3.1 g 22 mmol) in DMF (20 mL) was stirred for 30 minutes after which 1-(2-chloro-ethyl)-pyrrolidine (0.71 g, 4.2 mmol) was added. The mixture was heated to 50° C. for 6 hours, cooled to room temperature, filtered through a plug of silic...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ccc2n[nH]cc2c1
c1ccc2n[nH]cc2c1
c1ccc2n[nH]cc2c1.C1CC[NH]C1
HCl
CN(C)C=O
50
null
ClCCN1CCCC1.O=[N+]([O-])c1ccc2[nH]nc(Br)c2c1>CN(C)C=O>O=[N+]([O-])c1ccc2c(c1)c(Br)nn2CCN1CCCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ce051226ad6b4516a6a667311b4efcc1
O=[N+]([O-])c1ccc2c(c1)c(Br)nn2CCN1CCCC1>>Nc1ccc2c(c1)c(Br)nn2CCN1CCCC1
BrC1=NN(C2=CC=C(C=C12)[N+](=O)[O-])CCN1CCCC1.[Cl-].[NH4+]>>BrC1=NN(C2=CC=C(C=C12)N)CCN1CCCC1
O=[N+:1]([O-])[c:2]1[cH:3][cH:4][c:5]2[c:6]([cH:7]1)[c:8]([Br:9])[n:10][n:11]2[CH2:12][CH2:13][N:14]1[CH2:15][CH2:16][CH2:17][CH2:18]1>>[NH2:1][c:2]1[cH:3][cH:4][c:5]2[c:6]([cH:7]1)[c:8]([Br:9])[n:10][n:11]2[CH2:12][CH2:13][N:14]1[CH2:15][CH2:16][CH2:17][CH2:18]1
O=[N+]([O-])c1ccc2c(c1)c(Br)nn2CCN1CCCC1
Nc1ccc2c(c1)c(Br)nn2CCN1CCCC1
null
[Fe]
C(C)O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc2c(c1)cnn2CCN1CCCC1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
70
[{"value": 70.0, "product": "BrC1=NN(C2=CC=C(C=C12)N)CCN1CCCC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 69.3, "product": "BrC1=NN(C2=CC=C(C=C12)N)CCN1CCCC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
A mixture of 3-bromo-5-nitro-1-(2-pyrrolidin-1-yl-ethyl)-1H-indazole (1.9 g, 5.6 mmol), iron powder (3.1 g, 56 mmol), and ammonium chloride (0.15 g, 2.8 mmol) in 80% ethanol was heated to reflux for 3 hours, cooled to room temperature and concentrated under reduced pressure. The residue was taken up and stirred in trie...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccc2n[nH]cc2c1.C1CC[NH]C1
Other
[Fe].C(C)O
null
0.25
O=[N+]([O-])c1ccc2c(c1)c(Br)nn2CCN1CCCC1>[Fe].C(C)O>Nc1ccc2c(c1)c(Br)nn2CCN1CCCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-89fd0e5818a94079863ca5d75b90b759
ClCCN1CCCC1.O=[N+]([O-])c1ccc2c(Cl)n[nH]c2c1>>O=[N+]([O-])c1ccc2c(Cl)nn(CCN3CCCC3)c2c1
ClC1=NNC2=CC(=CC=C12)[N+](=O)[O-].C([O-])([O-])=O.[K+].[K+].ClCCN1CCCC1>>ClC1=NN(C2=CC(=CC=C12)[N+](=O)[O-])CCN1CCCC1
Cl[CH2:12][CH2:13][N:14]1[CH2:15][CH2:16][CH2:17][CH2:18]1.[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]2[c:8]([Cl:9])[n:10][nH:11][c:19]2[cH:20]1>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]2[c:8]([Cl:9])[n:10][n:11]([CH2:12][CH2:13][N:14]3[CH2:15][CH2:16][CH2:17][CH2:18]3)[c:19]2[cH:20]1
ClCCN1CCCC1.O=[N+]([O-])c1ccc2c(Cl)n[nH]c2c1
O=[N+]([O-])c1ccc2c(Cl)nn(CCN3CCCC3)c2c1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
61b0a224b62ca0b743a21f455645a524e1404d8b5e8bd813e0a3f8c6a5539082
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ccc2c(c1)cnn2CCN1CCCC1
Cl-[CH2;D2;+0:1]-[C:2]-[#7:3].[c:4]:[c:5]1:[c:6]:[c:7]:[#7;a:8]:[nH;D2;+0:9]:1>>[#7:3]-[C:2]-[CH2;D2;+0:1]-[n;H0;D3;+0:9]1:[#7;a:8]:[c:7]:[c:6]:[c:5]:1:[c:4]
66
[{"value": 66.0, "product": "ClC1=NN(C2=CC(=CC=C12)[N+](=O)[O-])CCN1CCCC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 65.0, "product": "ClC1=NN(C2=CC(=CC=C12)[N+](=O)[O-])CCN1CCCC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
50
CELSIUS
null
null
A mixture of 3-chloro-6-nitro-1H-indazole (2.4 g, 12 mmol) was treated with potassium carbonate (5.0 g, 36 mmol) in DMF (40 mL) for about 30 minutes, after which 1-(2-chloro-ethyl)-pyrrolidine (3.1 g, 18 mmol) was added. The mixture was heated to 50° C. for 6 hours, cooled to room temperature and filtered through a plu...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ccc2n[nH]cc2c1
c1ccc2c[nH]nc2c1
c1ccc2c[nH]nc2c1.C1CC[NH]C1
HCl
CN(C)C=O
50
null
ClCCN1CCCC1.O=[N+]([O-])c1ccc2c(Cl)n[nH]c2c1>CN(C)C=O>O=[N+]([O-])c1ccc2c(Cl)nn(CCN3CCCC3)c2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-91125852705c46c2ac65ca624730bb73
O=[N+]([O-])c1ccc2c(Cl)nn(CCN3CCCC3)c2c1>>Nc1ccc2c(Cl)nn(CCN3CCCC3)c2c1
ClC1=NN(C2=CC(=CC=C12)[N+](=O)[O-])CCN1CCCC1.[Cl-].[NH4+]>>ClC1=NN(C2=CC(=CC=C12)N)CCN1CCCC1
O=[N+:1]([O-])[c:2]1[cH:3][cH:4][c:5]2[c:6]([Cl:7])[n:8][n:9]([CH2:10][CH2:11][N:12]3[CH2:13][CH2:14][CH2:15][CH2:16]3)[c:17]2[cH:18]1>>[NH2:1][c:2]1[cH:3][cH:4][c:5]2[c:6]([Cl:7])[n:8][n:9]([CH2:10][CH2:11][N:12]3[CH2:13][CH2:14][CH2:15][CH2:16]3)[c:17]2[cH:18]1
O=[N+]([O-])c1ccc2c(Cl)nn(CCN3CCCC3)c2c1
Nc1ccc2c(Cl)nn(CCN3CCCC3)c2c1
null
[Fe]
C(C)O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc2c(c1)cnn2CCN1CCCC1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]:[c:5]:[#7;a:6]>>[#7;a:6]:[c:5]:[c:4]:[c:2](-[NH2;D1;+0:1]):[c:3]
82.3
[{"value": 80.0, "product": "ClC1=NN(C2=CC(=CC=C12)N)CCN1CCCC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 82.3, "product": "ClC1=NN(C2=CC(=CC=C12)N)CCN1CCCC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
A mixture of 3-chloro-6-nitro-1-(2-pyrrolidin-1-yl-ethyl)-1H-indazole (2.3 g, 7.8 mmol), iron powder (3.5 g, 62 mmol), and ammonium chloride (0.21 g, 3.9 mmol) in 80% Ethanol was heated to reflux for 3 hours, cooled to room temperature, and concentrated under reduced pressure. The residue was stirred in triethylamine/e...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccc2c[nH]nc2c1.C1CC[NH]C1
Other
[Fe].C(C)O
null
0.25
O=[N+]([O-])c1ccc2c(Cl)nn(CCN3CCCC3)c2c1>[Fe].C(C)O>Nc1ccc2c(Cl)nn(CCN3CCCC3)c2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c2b7d8d1070148d98a5ad00d051f22d2
O=[N+]([O-])c1ccc2cn[nH]c2c1.[Br-]>>O=[N+]([O-])c1ccc2c(Br)n[nH]c2c1
Cl.[N+](=O)([O-])C1=CC=C2C=NNC2=C1.[OH-].[Na+].[Br-].[Br-].[Br-].[NH+]1=CC=CC=C1.[NH+]1=CC=CC=C1.[NH+]1=CC=CC=C1>>BrC1=NNC2=CC(=CC=C12)[N+](=O)[O-]
[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]2[cH:8][n:10][nH:11][c:12]2[cH:13]1.[Br-:9]>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]2[c:8]([Br:9])[n:10][nH:11][c:12]2[cH:13]1
O=[N+]([O-])c1ccc2cn[nH]c2c1.[Br-]
O=[N+]([O-])c1ccc2c(Br)n[nH]c2c1
null
null
O.CO
Functional Group Interconversion
Bromination
35e4f92aa8c0c274f67627ca98b5ec6bde8d1693193a68ce34b02032f7360dd9
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1ccc2[nH]ncc2c1
[Br-;H0;D0:1].[c:2]:[c:3]1:[#7;a:4]:[#7;a:5]:[cH;D2;+0:6]:[c:7]:1:[c:8]>>[Br;H0;D1;+0:1]-[c;H0;D3;+0:6]1:[#7;a:5]:[#7;a:4]:[c:3](:[c:2]):[c:7]:1:[c:8]
null
[]
0
CELSIUS
15
MINUTE
A mixture of NaOH (2.0 g, 50 mmol) in H2O (60 mL) was added 6-nitroindazole (2.0 g, 12 mmol) and the suspension heated until a red solution formed. The mixture was placed in an ice-water bath for 15 minutes after which pyridinium tribromide (4.7 g, 15 mmol) in MeOH (15 mL) was added. The mixture was stirred at 0° C. fo...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2n[nH]cc2c1
c1ccc2n[nH]cc2c1
c1ccc2n[nH]cc2c1
null
O.CO
0
0.25
O=[N+]([O-])c1ccc2cn[nH]c2c1.[Br-]>O.CO>O=[N+]([O-])c1ccc2c(Br)n[nH]c2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d525da7ec79f45ea8aa85457cb1368cd
ClCCN1CCCC1.O=[N+]([O-])c1ccc2c(Br)n[nH]c2c1>>O=[N+]([O-])c1ccc2c(Br)nn(CCN3CCCC3)c2c1
BrC1=NNC2=CC(=CC=C12)[N+](=O)[O-].C([O-])([O-])=O.[K+].[K+].ClCCN1CCCC1>>BrC1=NN(C2=CC(=CC=C12)[N+](=O)[O-])CCN1CCCC1
Cl[CH2:12][CH2:13][N:14]1[CH2:15][CH2:16][CH2:17][CH2:18]1.[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]2[c:8]([Br:9])[n:10][nH:11][c:19]2[cH:20]1>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]2[c:8]([Br:9])[n:10][n:11]([CH2:12][CH2:13][N:14]3[CH2:15][CH2:16][CH2:17][CH2:18]3)[c:19]2[cH:20]1
ClCCN1CCCC1.O=[N+]([O-])c1ccc2c(Br)n[nH]c2c1
O=[N+]([O-])c1ccc2c(Br)nn(CCN3CCCC3)c2c1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
61b0a224b62ca0b743a21f455645a524e1404d8b5e8bd813e0a3f8c6a5539082
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ccc2c(c1)cnn2CCN1CCCC1
Cl-[CH2;D2;+0:1]-[C:2]-[#7:3].[c:4]:[c:5]1:[c:6]:[c:7]:[#7;a:8]:[nH;D2;+0:9]:1>>[#7:3]-[C:2]-[CH2;D2;+0:1]-[n;H0;D3;+0:9]1:[#7;a:8]:[c:7]:[c:6]:[c:5]:1:[c:4]
64.7
[{"value": 64.0, "product": "BrC1=NN(C2=CC(=CC=C12)[N+](=O)[O-])CCN1CCCC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 64.7, "product": "BrC1=NN(C2=CC(=CC=C12)[N+](=O)[O-])CCN1CCCC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
50
CELSIUS
null
null
A mixture of 3-bromo-6-nitro-1H-indazole (1.0 g, 4.1 mmol) and potassium carbonate (2.9 g 21 mmol) in DMF (20 mL) was stirred for 30 minutes after which 1-(2-chloro-ethyl)-pyrrolidine (1.8 g, 10 mmol) was added. The mixture was heated to 50° C. for 6 hours, cooled to room temperature and filtered through a plug of sili...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ccc2n[nH]cc2c1
c1ccc2c[nH]nc2c1
c1ccc2c[nH]nc2c1.C1CC[NH]C1
HCl
CN(C)C=O
50
null
ClCCN1CCCC1.O=[N+]([O-])c1ccc2c(Br)n[nH]c2c1>CN(C)C=O>O=[N+]([O-])c1ccc2c(Br)nn(CCN3CCCC3)c2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-82339a0c5f9a4a9eb8ee8a1ec45299e4
O=[N+]([O-])c1ccc2c(Br)nn(CCN3CCCC3)c2c1>>Nc1ccc2c(Br)nn(CCN3CCCC3)c2c1
BrC1=NN(C2=CC(=CC=C12)[N+](=O)[O-])CCN1CCCC1.[Cl-].[NH4+]>>BrC1=NN(C2=CC(=CC=C12)N)CCN1CCCC1
O=[N+:1]([O-])[c:2]1[cH:3][cH:4][c:5]2[c:6]([Br:7])[n:8][n:9]([CH2:10][CH2:11][N:12]3[CH2:13][CH2:14][CH2:15][CH2:16]3)[c:17]2[cH:18]1>>[NH2:1][c:2]1[cH:3][cH:4][c:5]2[c:6]([Br:7])[n:8][n:9]([CH2:10][CH2:11][N:12]3[CH2:13][CH2:14][CH2:15][CH2:16]3)[c:17]2[cH:18]1
O=[N+]([O-])c1ccc2c(Br)nn(CCN3CCCC3)c2c1
Nc1ccc2c(Br)nn(CCN3CCCC3)c2c1
null
[Fe]
C(C)O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc2c(c1)cnn2CCN1CCCC1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]:[c:5]:[#7;a:6]>>[#7;a:6]:[c:5]:[c:4]:[c:2](-[NH2;D1;+0:1]):[c:3]
95
[{"value": 95.0, "product": "BrC1=NN(C2=CC(=CC=C12)N)CCN1CCCC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 93.4, "product": "BrC1=NN(C2=CC(=CC=C12)N)CCN1CCCC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
A mixture of 3-bromo-6-nitro-1-(2-pyrrolidin-1-yl-ethyl)-1H-indazole (0.90 g, 2.7 mmol), iron powder (1.5 g, 26 mmol), and ammonium chloride (73 mg, 1.3 mmol) in 80% ethanol was heated to reflux for 3 hours, cooled to room temperature and concentrated under reduced pressure. The residue was taken up and stirred in trie...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccc2c[nH]nc2c1.C1CC[NH]C1
Other
[Fe].C(C)O
null
0.25
O=[N+]([O-])c1ccc2c(Br)nn(CCN3CCCC3)c2c1>[Fe].C(C)O>Nc1ccc2c(Br)nn(CCN3CCCC3)c2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4aea544eff374c7797839e5e5d48937d
CC(=O)C(C)=O.Nc1ccc2c(cnn2CCN2CCCC2)c1>>COC(CNc1ccc2c(cnn2CCN2CCCC2)c1)OC
[BH-](OC(=O)C)(OC(=O)C)OC(=O)C.[Na+].[BH-](OC(=O)C)(OC(=O)C)OC(=O)C.[Na+].C1CCOC1.N1(CCCC1)CCN1N=CC2=CC(=CC=C12)N.CC(C(=O)C)=O.C1CCOC1>>COC(CNC=1C=C2C=NN(C2=CC1)CCN1CCCC1)OC
CC(=O)[C:3]([CH3:4])=[O:22].[NH2:5][c:6]1[cH:7][cH:8][c:9]2[c:10]([cH:11][n:12][n:13]2[CH2:14][CH2:15][N:16]2[CH2:17][CH2:18][CH2:19][CH2:20]2)[cH:21]1>>[CH3:1][O:2][CH:3]([CH2:4][NH:5][c:6]1[cH:7][cH:8][c:9]2[c:10]([cH:11][n:12][n:13]2[CH2:14][CH2:15][N:16]2[CH2:17][CH2:18][CH2:19][CH2:20]2)[cH:21]1)[O:22][CH3:23]
CC(=O)C(C)=O.Nc1ccc2c(cnn2CCN2CCCC2)c1
COC(CNc1ccc2c(cnn2CCN2CCCC2)c1)OC
null
null
CC(C)(C)OC
Heteroatom Alkylation and Arylation
OtherReaction
87896795e963146046544ee0cde49480e26b3c18871424d315206a364e0f56a4
becaaaecd78523328db920a0fe4df620e3cea197aaac9805e376373b3c66faa1
c1ccc2c(c1)cnn2CCN1CCCC1
C-C(=O)-[C;H0;D3;+0:1](-[CH3;D1;+0:2])=[O;H0;D1;+0:3].[NH2;D1;+0:4]-[c:5](:[c:6]):[c:7]>>[C;D1;H3:8]-[#8:9]-[CH;D3;+0:1](-[CH2;D2;+0:2]-[NH;D2;+0:4]-[c:5](:[c:6]):[c:7])-[O;H0;D2;+0:3]-[C;D1;H3:10]
null
[]
null
null
12
HOUR
To a solution of 1-(2-pyrrolidin-1-yl-ethyl)-1H-indazol-5-ylamine (1.14 g, 0.497 mmol) in 62 mL of dry THF was added 2.04 mL of dimethyl glyoxal in MTBE (45% glyoxal by weight). A slurry of NaBH(OAc)3 (1.66 g, 7.83 mmol) in THF (10 mL) was slowly added via addition funnel over 60 minutes, and the mixture stirred at roo...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ketone.Primary amine
Ether.Ether.Secondary amine
null
null
c1ccc2n[nH]cc2c1.C1CC[NH]C1
null
CC(C)(C)OC
null
12
CC(=O)C(C)=O.Nc1ccc2c(cnn2CCN2CCCC2)c1>CC(C)(C)OC>COC(CNc1ccc2c(cnn2CCN2CCCC2)c1)OC
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-84c8be1d487f4a98ba71233dc7b69f16
O=c1n(-c2ccc(Oc3ccccc3)cc2)ccn1-c1ccc2c(cnn2CCN2CCCC2)c1>>O=C1N(c2ccc(Oc3ccccc3)cc2)CCN1c1ccc2c(cnn2CCN2CCCC2)c1
O(C1=CC=CC=C1)C1=CC=C(C=C1)N1C(N(C=C1)C=1C=C2C=NN(C2=CC1)CCN1CCCC1)=O.[H][H]>>O(C1=CC=CC=C1)C1=CC=C(C=C1)N1C(N(CC1)C=1C=C2C=NN(C2=CC1)CCN1CCCC1)=O
[O:1]=[c:2]1[n:3](-[c:4]2[cH:5][cH:6][c:7]([O:8][c:9]3[cH:10][cH:11][cH:12][cH:13][cH:14]3)[cH:15][cH:16]2)[cH:17][cH:18][n:19]1-[c:20]1[cH:21][cH:22][c:23]2[c:24]([cH:25][n:26][n:27]2[CH2:28][CH2:29][N:30]2[CH2:31][CH2:32][CH2:33][CH2:34]2)[cH:35]1>>[O:1]=[C:2]1[N:3]([c:4]2[cH:5][cH:6][c:7]([O:8][c:9]3[cH:10][cH:11][c...
O=c1n(-c2ccc(Oc3ccccc3)cc2)ccn1-c1ccc2c(cnn2CCN2CCCC2)c1
O=C1N(c2ccc(Oc3ccccc3)cc2)CCN1c1ccc2c(cnn2CCN2CCCC2)c1
null
[Pd]
CC(=O)O
Reduction
OtherReaction
02d4454334aa6aefae7f49d82f12172420ac9a0dc7c46e64c030ab4763c359b1
80a720e2607cb3e63102e764b72ebf8ab153bd656e5e1870bdae6ef44ada08f6
O=C1N(c2ccc(Oc3ccccc3)cc2)CCN1c1ccc2c(cnn2CCN2CCCC2)c1
[O;D1;H0:1]=[c;H0;D3;+0:2]1:[n;H0;D3;+0:3](-[c;H0;D3;+0:4]2:[c:5]:[c:6]:[c:7]3:[#7;a:8]:[#7;a:9]:[c:10]:[c:11]:3:[c:12]:2):[cH;D2;+0:13]:[cH;D2;+0:14]:[n;H0;D3;+0:15]:1-[c;H0;D3;+0:16](:[c:17]:[c:18]):[c:19]:[c:20]>>[O;D1;H0:1]=[C;H0;D3;+0:2]1-[N;H0;D3;+0:3](-[c;H0;D3;+0:4]2:[c:5]:[c:6]:[c:7]3:[#7;a:8]:[#7;a:9]:[c:10]:...
null
[]
null
null
6
HOUR
1-(4-phenoxyphenyl)-3-[1-(2-pyrrolidin-1-ylethyl)-1H-indazol-5-yl]-1,3-dihydro-2H-imidazol-2-one (Example 118) (0.100 g, 0.215 mmol) was dissolved in 20 mL of AcOH and 100 mg of Pd/C (10% mol/mol) was added. The mixture was subjected to an atmosphere of hydrogen gas at a pressure of 60 psi in a Parr shaker apparatus, a...
10.6084/m9.figshare.5104873.v1
null
null
Urea
c1ncc[nH]1
C1C[NH]C[NH]1
C1C[NH]C[NH]1.c1ccccc1.c1ccccc1.c1ccc2n[nH]cc2c1.C1CC[NH]C1
null
[Pd].CC(=O)O
null
6
O=c1n(-c2ccc(Oc3ccccc3)cc2)ccn1-c1ccc2c(cnn2CCN2CCCC2)c1>[Pd].CC(=O)O>O=C1N(c2ccc(Oc3ccccc3)cc2)CCN1c1ccc2c(cnn2CCN2CCCC2)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c9b3ff3d6bf246c4a792e741974357f7
Nc1ccc(CCCC(=O)O)cc1>>O=C1NC(=O)c2ccccc21
NC1=CC=C(C=C1)CCCC(=O)O.C(C)N(CC)CC.CN(C)C1=NC=CC=C1.C(C(C)O)O>>C1(C=2C(C(N1)=O)=CC=CC2)=O
C(C[CH2:9][c:8]1[cH:7][cH:6][c:4]([NH2:3])[cH:11][cH:10]1)[C:2](=[O:1])[OH:5]>>[O:1]=[C:2]1[NH:3][C:4](=[O:5])[c:6]2[cH:7][cH:8][cH:9][cH:10][c:11]21
Nc1ccc(CCCC(=O)O)cc1
O=C1NC(=O)c2ccccc21
null
null
O
Aromatic Heterocycle Formation
OtherReaction
9f8eb762b61e31b1c74f37004bc2b68f2e2ba32dacd41072d219be9b2d4c78ea
969319f6b6b635c4fd197991279ae7a2965391dd6ffca4bfef8c9fe1acfc0d65
O=C1NC(=O)c2ccccc21
[NH2;D1;+0:1]-[c;H0;D3;+0:2]1:[cH;D2;+0:3]:[cH;D2;+0:4]:[c;H0;D3;+0:5](-[CH2;D2;+0:6]-C-C-[C;H0;D3;+0:7](=[O;D1;H0:8])-[OH;D1;+0:9]):[c:10]:[cH;D2;+0:11]:1>>[O;D1;H0:8]=[C;H0;D3;+0:7]1-[NH;D2;+0:1]-[C;H0;D3;+0:2](=[O;H0;D1;+0:9])-[c;H0;D3;+0:11]2:[c:10]:[cH;D2;+0:5]:[cH;D2;+0:6]:[cH;D2;+0:4]:[c;H0;D3;+0:3]:2-1
null
[]
140
CELSIUS
330
MINUTE
A suspension of 2.40 g (16.3 mmol) and 2.80 g (15.6 mmol) of 4-(4aminophenyl)butyric acid in 20 mL of propylene glycol, 2.40 mL (1.74 g, 17.3 mmol) of triethylamine and 10 mg (0.08 mmol) of dimethylaminopyridine was heated to 140° C. The mixture became a clear solution after 5 min at 140° C. After stirring for 330 min,...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Unsubstituted dicarboximide
c1ccccc1
c1ccc2c(c1)CNC2
c1ccc2c(c1)CNC2
Other
O
140
5.5
Nc1ccc(CCCC(=O)O)cc1>O>O=C1NC(=O)c2ccccc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-58b3cb8204414646ad140d3448e846a9
NO.Nc1ccc2ncsc2c1.O=CC(Cl)(Cl)Cl>>O=C(C=NO)Nc1ccc2ncsc2c1
NC1=CC2=C(N=CS2)C=C1.Cl.ON.S(=O)(=O)([O-])[O-].[Na+].[Na+].O=CC(Cl)(Cl)Cl>>S1C=NC2=C1C=C(C=C2)NC(C=NO)=O
[NH2:4][OH:5].[NH2:6][c:7]1[cH:8][cH:9][c:10]2[n:11][cH:12][s:13][c:14]2[cH:15]1.Cl[C:2](Cl)(Cl)[CH:3]=[O:1]>>[O:1]=[C:2]([CH:3]=[N:4][OH:5])[NH:6][c:7]1[cH:8][cH:9][c:10]2[n:11][cH:12][s:13][c:14]2[cH:15]1
NO.Nc1ccc2ncsc2c1.O=CC(Cl)(Cl)Cl
O=C(C=NO)Nc1ccc2ncsc2c1
null
null
Cl.O.C(C)O
Acylation
OtherReaction
a5f86f1d718ab7ac00a957b033bada788dadb0950aa0d34d7e24a73a42d26116
d29015920ce18914ddb4669715a8994e1383d81f1a08fa7e118fc3458ea45afa
c1ccc2scnc2c1
Cl-[C;H0;D4;+0:1](-Cl)(-Cl)-[CH;D2;+0:2]=[O;H0;D1;+0:3].[#16;a:4]:[c:5]:[c:6]:[c:7](-[NH2;D1;+0:8]):[c:9].[NH2;D1;+0:10]-[O;D1;H1:11]>>[#16;a:4]:[c:5]:[c:6]:[c:7](-[NH;D2;+0:8]-[C;H0;D3;+0:1](=[O;H0;D1;+0:3])-[CH;D2;+0:2]=[N;H0;D2;+0:10]-[O;D1;H1:11]):[c:9]
94
[{"value": 94.0, "product": "S1C=NC2=C1C=C(C=C2)NC(C=NO)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
To a 1-L flask was added a magnetic stir bar, 85 g of sodium sulfate, and 100 mL of water. The mixture was magnetically stirred until all the solids were dissolved. To the resultant aqueous solution was added a solution of 6-aminobenzothiazole (4.96 g, 33.0 mmol) in 50 mL of 1N aqueous hydrochloric acid and 10 mL of et...
10.6084/m9.figshare.5104873.v1
null
Trichloro group.Aldehyde.Primary amine.Primary amine
Secondary amide.Oxime
null
null
c1ccc2scnc2c1
HCl
Cl.O.C(C)O
null
0.25
NO.Nc1ccc2ncsc2c1.O=CC(Cl)(Cl)Cl>Cl.O.C(C)O>O=C(C=NO)Nc1ccc2ncsc2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-08d169f88caf407d99825c179a1e5d3c
O=C(C=NO)Nc1ccc2ncsc2c1>>O=C1Nc2ccc3ncsc3c2C1=O
S(O)(O)(=O)=O.S(O)(O)(=O)=O.S1C=NC2=C1C=C(C=C2)NC(C=NO)=O>>S1C=NC2=CC=C3NC(C(C3=C12)=O)=O
N(=[CH:13][C:2](=[O:1])[NH:3][c:4]1[cH:5][cH:6][c:7]2[n:8][cH:9][s:10][c:11]2[cH:12]1)[OH:14]>>[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][c:7]3[n:8][cH:9][s:10][c:11]3[c:12]2[C:13]1=[O:14]
O=C(C=NO)Nc1ccc2ncsc2c1
O=C1Nc2ccc3ncsc3c2C1=O
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
76ca54020825c2b52c69b966e96a6ad71d1ab32767482feb664c3cb4ea38d255
ab4bf08516e66cf6fd8670ac9e8d4ecd074b35f40b66b51c2d0c9c0d98ab1c51
O=C1Nc2ccc3ncsc3c2C1=O
[O;D1;H0:1]=[C:2](-[#7:3]-[c:4]1:[c:5]:[c:6]:[c:7]2:[#7;a:8]:[c:9]:[#16;a:10]:[c:11]:2:[cH;D2;+0:12]:1)-[CH;D2;+0:13]=N-[OH;D1;+0:14]>>[O;D1;H0:1]=[C:2]1-[#7:3]-[c:4]2:[c:5]:[c:6]:[c:7]3:[#7;a:8]:[c:9]:[#16;a:10]:[c:11]:3:[c;H0;D3;+0:12]:2-[C;H0;D3;+0:13]-1=[O;H0;D1;+0:14]
46
[{"value": 46.0, "product": "S1C=NC2=CC=C3NC(C(C3=C12)=O)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a 1-L flask was added a magnetic stir bar, 85 g of sodium sulfate, and 100 mL of water. The mixture was magnetically stirred until all the solids were dissolved. To the resultant aqueous solution was added a solution of 6-aminobenzothiazole (4.96 g, 33.0 mmol) in 50 mL of 1N aqueous hydrochloric acid and 10 mL of et...
10.6084/m9.figshare.5104873.v1
null
Oxime
Ketone
c1ccc2scnc2c1
c1nc2ccc3c(c2s1)CCN3
c1nc2ccc3c(c2s1)CCN3
Other
O
null
1
O=C(C=NO)Nc1ccc2ncsc2c1>O>O=C1Nc2ccc3ncsc3c2C1=O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f0c12e893fac446f907a14ce49c4c16b
CS(=O)(=O)Nc1ccc(N)cc1.O=C1Nc2ccccc2C1=CO>>CS(=O)(=O)Nc1ccc(N/C=C2\C(=O)Nc3ccccc32)cc1
OC=C1C(NC2=CC=CC=C12)=O.NC1=CC=C(C=C1)NS(=O)(=O)C>>O=C\1NC2=CC=CC=C2/C1=C/NC1=CC=C(C=C1)NS(=O)(=O)C
[CH3:1][S:2](=[O:3])(=[O:4])[NH:5][c:6]1[cH:7][cH:8][c:9]([NH2:10])[cH:22][cH:23]1.O[CH:11]=[C:12]1[C:13](=[O:14])[NH:15][c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]21>>[CH3:1][S:2](=[O:3])(=[O:4])[NH:5][c:6]1[cH:7][cH:8][c:9]([NH:10]/[CH:11]=[C:12]2\[C:13](=[O:14])[NH:15][c:16]3[cH:17][cH:18][cH:19][cH:20][c:21]32)[cH:22...
CS(=O)(=O)Nc1ccc(N)cc1.O=C1Nc2ccccc2C1=CO
CS(=O)(=O)Nc1ccc(N/C=C2\C(=O)Nc3ccccc32)cc1
null
null
null
Heteroatom Alkylation and Arylation
Reductive amination with alcohol
ac661a5987df49e763a2386679221354b73376953f4071e32e52e2d7e8877593
dc27e5e3871ba014ddcdbe66aa8244518b94cc851f1ff4159b6674656bc3b780
O=C1Nc2ccccc2/C1=C/Nc1ccccc1
O-[CH;D2;+0:1]=[C:2]1-[c:3]:[c:4]-[#7:5]-[C:6]-1=[O;D1;H0:7].[NH2;D1;+0:8]-[c:9](:[c:10]):[c:11]>>[O;D1;H0:7]=[C:6]1-[#7:5]-[c:4]:[c:3]/[C:2]-1=[CH;D2;+0:1]/[NH;D2;+0:8]-[c:9](:[c:10]):[c:11]
null
[]
null
null
null
null
The title compound was prepared analogous to Example 5 from 3-(hydroxymethylene)-1,3-dihydro-2H-indol-2-one (0.164 g, 1.02 mmol) and N-(4-aminophenyl)-methanesulfonamide [53250-82-1, 0.186 g, 1.0 mmol] to provide a yellow solid (0.249 g). 1H NMR (DMSO) 10.67 (d, 1H); 10.45 (s, 1H); 9.56 (s, 1H); 8.50 (d, 1H); 7.52 (d, ...
10.6084/m9.figshare.5104873.v1
null
Enol.Primary amine
Enamine
null
null
c1ccccc1.c1ccc2c(c1)CCN2
HO-
null
null
null
CS(=O)(=O)Nc1ccc(N)cc1.O=C1Nc2ccccc2C1=CO>>CS(=O)(=O)Nc1ccc(N/C=C2\C(=O)Nc3ccccc32)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-99b7a8779cde4571a68bccdeba305e57
Nc1ccc(S(=O)(=O)Nc2ccccn2)cc1.O=C1Nc2ccccc2C1=CO>>O=C1Nc2ccccc2/C1=C/Nc1ccc(S(=O)(=O)Nc2ccccn2)cc1
OC=C1C(NC2=CC=CC=C12)=O.C=1C=CN=C(C1)NS(=O)(=O)C=2C=CC(=CC2)N>>O=C\1NC2=CC=CC=C2/C1=C/NC1=CC=C(C=C1)S(=O)(=O)NC1=NC=CC=C1
[NH2:12][c:13]1[cH:14][cH:15][c:16]([S:17](=[O:18])(=[O:19])[NH:20][c:21]2[cH:22][cH:23][cH:24][cH:25][n:26]2)[cH:27][cH:28]1.O[CH:11]=[C:10]1[C:2](=[O:1])[NH:3][c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]21>>[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2/[C:10]1=[CH:11]/[NH:12][c:13]1[cH:14][cH:15][c:16]([S:17](=[O:18]...
Nc1ccc(S(=O)(=O)Nc2ccccn2)cc1.O=C1Nc2ccccc2C1=CO
O=C1Nc2ccccc2/C1=C/Nc1ccc(S(=O)(=O)Nc2ccccn2)cc1
null
null
null
Heteroatom Alkylation and Arylation
Reductive amination with alcohol
ac661a5987df49e763a2386679221354b73376953f4071e32e52e2d7e8877593
dc27e5e3871ba014ddcdbe66aa8244518b94cc851f1ff4159b6674656bc3b780
O=C1Nc2ccccc2/C1=C/Nc1ccc(S(=O)(=O)Nc2ccccn2)cc1
O-[CH;D2;+0:1]=[C:2]1-[c:3]:[c:4]-[#7:5]-[C:6]-1=[O;D1;H0:7].[NH2;D1;+0:8]-[c:9](:[c:10]):[c:11]>>[O;D1;H0:7]=[C:6]1-[#7:5]-[c:4]:[c:3]/[C:2]-1=[CH;D2;+0:1]/[NH;D2;+0:8]-[c:9](:[c:10]):[c:11]
null
[]
null
null
null
null
The title compound was prepared analogous to Example 5 from 3-(hydroxymethylene)-1,3-dihydro-2H-indol-2-one and sulfapyridine. Electrospray MS 393 (MH+). Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Enol.Primary amine
Enamine
null
null
c1ccc2c(c1)CCN2.c1ccccc1.c1ccncc1
HO-
null
null
null
Nc1ccc(S(=O)(=O)Nc2ccccn2)cc1.O=C1Nc2ccccc2C1=CO>>O=C1Nc2ccccc2/C1=C/Nc1ccc(S(=O)(=O)Nc2ccccn2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-346e2a2df06741239ca7c06c272f201f
Cc1nnc(NS(=O)(=O)c2ccc(N)cc2)s1.O=C1Nc2ccccc2C1=CO>>Cc1nnc(NS(=O)(=O)c2ccc(N/C=C3\C(=O)Nc4ccccc43)cc2)s1
OC=C1C(NC2=CC=CC=C12)=O.NC1=CC=C(C=C1)S(=O)(=O)NC=1SC(=NN1)C>>CC1=NN=C(S1)NS(=O)(=O)C1=CC=C(C=C1)N\C=C\1/C(NC2=CC=CC=C12)=O
[CH3:1][c:2]1[n:3][n:4][c:5]([NH:6][S:7](=[O:8])(=[O:9])[c:10]2[cH:11][cH:12][c:13]([NH2:14])[cH:26][cH:27]2)[s:28]1.O[CH:15]=[C:16]1[C:17](=[O:18])[NH:19][c:20]2[cH:21][cH:22][cH:23][cH:24][c:25]21>>[CH3:1][c:2]1[n:3][n:4][c:5]([NH:6][S:7](=[O:8])(=[O:9])[c:10]2[cH:11][cH:12][c:13]([NH:14]/[CH:15]=[C:16]3\[C:17](=[O:1...
Cc1nnc(NS(=O)(=O)c2ccc(N)cc2)s1.O=C1Nc2ccccc2C1=CO
Cc1nnc(NS(=O)(=O)c2ccc(N/C=C3\C(=O)Nc4ccccc43)cc2)s1
null
null
null
Heteroatom Alkylation and Arylation
Reductive amination with alcohol
ac661a5987df49e763a2386679221354b73376953f4071e32e52e2d7e8877593
dc27e5e3871ba014ddcdbe66aa8244518b94cc851f1ff4159b6674656bc3b780
O=C1Nc2ccccc2/C1=C/Nc1ccc(S(=O)(=O)Nc2nncs2)cc1
O-[CH;D2;+0:1]=[C:2]1-[c:3]:[c:4]-[#7:5]-[C:6]-1=[O;D1;H0:7].[NH2;D1;+0:8]-[c:9](:[c:10]):[c:11]>>[O;D1;H0:7]=[C:6]1-[#7:5]-[c:4]:[c:3]/[C:2]-1=[CH;D2;+0:1]/[NH;D2;+0:8]-[c:9](:[c:10]):[c:11]
null
[]
null
null
null
null
The title compound was prepared analogous to Example 5 from 3-(hydroxymethylene)-1,3-dihydro-2H-indol-2-one and 4-amino-N-(5-methyl[1,3,4]thiadiazol-2-yl)-benzenesulfonamide. 1H NMR (DMSO) 13.90 (bs, 1H); 10.84 (d, 1H); 10.58 (s, 1H); 8.62 (d, 1H); 7.81 (d, 2H); 7.60 (d, 1H); 7.55 (d, 2H); 7.12 (m, 1H); 6.95 (m, 1H); 7...
10.6084/m9.figshare.5104873.v1
null
Enol.Primary amine
Enamine
null
null
c1nncs1.c1ccccc1.c1ccc2c(c1)CCN2
HO-
null
null
null
Cc1nnc(NS(=O)(=O)c2ccc(N)cc2)s1.O=C1Nc2ccccc2C1=CO>>Cc1nnc(NS(=O)(=O)c2ccc(N/C=C3\C(=O)Nc4ccccc43)cc2)s1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5a54b51f05384a30bd1356871b0a78f2
COc1ccc(C=O)cc1Br.Cc1cc2c(cc1B(O)O)C(C)(C)CCC2(C)C>>COc1ccc(C=O)cc1-c1cc2c(cc1C)C(C)(C)CCC2(C)C
BrC=1C=C(C=O)C=CC1OC.CC=1C(=CC=2C(CCC(C2C1)(C)C)(C)C)B(O)O.C([O-])([O-])=O.[K+].[K+]>>CC=1C(=CC=2C(CCC(C2C1)(C)C)(C)C)C=1C=C(C=O)C=CC1OC
Br[c:10]1[c:3]([O:2][CH3:1])[cH:4][cH:5][c:6]([CH:7]=[O:8])[cH:9]1.OB(O)[c:11]1[cH:12][c:13]2[c:14]([cH:15][c:16]1[CH3:17])[C:18]([CH3:19])([CH3:20])[CH2:21][CH2:22][C:23]2([CH3:24])[CH3:25]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH:7]=[O:8])[cH:9][c:10]1-[c:11]1[cH:12][c:13]2[c:14]([cH:15][c:16]1[CH3:17])[C:18]([CH3:19...
COc1ccc(C=O)cc1Br.Cc1cc2c(cc1B(O)O)C(C)(C)CCC2(C)C
COc1ccc(C=O)cc1-c1cc2c(cc1C)C(C)(C)CCC2(C)C
null
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1
O.COCCOC.C(C)(=O)OCC
C-C Coupling
Suzuki coupling with boronic acids
b6fa867d6aba2bef80ed68dbf682dd3adb3006465de50d2f754372d7f6e007ef
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc3c(c2)CCCC3)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]-[C:4]=[O;D1;H0:5]):[c:6](-[#8:7]):[c:8].O-B(-O)-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12](-[C;D1;H3:13]):[c:14]>>[#8:7]-[c:6](:[c:8]):[c;H0;D3;+0:1](-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:12](-[C;D1;H3:13]):[c:14]):[c:2]:[c:3]-[C:4]=[O;D1;H0:5]
90.1
[{"value": 90.0, "product": "CC=1C(=CC=2C(CCC(C2C1)(C)C)(C)C)C=1C=C(C=O)C=CC1OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 90.1, "product": "CC=1C(=CC=2C(CCC(C2C1)(C)C)(C)C)C=1C=C(C=O)C=CC1OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 3-bromo-4-methoxybenzaldehyde (19.0 g, 88.4 mmol), (3,5,5,8,8-pentamethyl-5,6,7,8-tetrahydronaphthalen-2-yl) boronic acid (23.8 g, 97.2 mmol) and potassium carbonate (48.8 g, 353.6 mmol) in 1,2-dimethoxyethane (500 mL) and water (40 mL) was degassed with argon for 60 minutes. Tetrakis(triphenylphosphine) p...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccc2c(c1)CCCC2
c1ccccc1.c1ccc2c(c1)CCCC2
c1ccccc1.c1ccc2c(c1)CCCC2
HBr.B
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.O.COCCOC.C(C)(=O)OCC
null
null
COc1ccc(C=O)cc1Br.Cc1cc2c(cc1B(O)O)C(C)(C)CCC2(C)C>[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.O.COCCOC.C(C)(=O)OCC>COc1ccc(C=O)cc1-c1cc2c(cc1C)C(C)(C)CCC2(C)C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a0c6cd4e3c5d49158be4f08f4d61f8d3
O=C1CCC(=O)N1Br.O=Cc1ccc(OC(F)(F)F)cc1>>O=Cc1ccc(OC(F)(F)F)c(Br)c1
BrN1C(CCC1=O)=O.FC(OC1=CC=C(C=O)C=C1)(F)F.C(Cl)Cl.OS(=O)(=O)O>>BrC=1C=C(C=O)C=CC1OC(F)(F)F
O=C1CCC(=O)N1[Br:13].[O:1]=[CH:2][c:3]1[cH:4][cH:5][c:6]([O:7][C:8]([F:9])([F:10])[F:11])[cH:12][cH:14]1>>[O:1]=[CH:2][c:3]1[cH:4][cH:5][c:6]([O:7][C:8]([F:9])([F:10])[F:11])[c:12]([Br:13])[cH:14]1
O=C1CCC(=O)N1Br.O=Cc1ccc(OC(F)(F)F)cc1
O=Cc1ccc(OC(F)(F)F)c(Br)c1
null
null
C(=O)(C(F)(F)F)O
Functional Group Interconversion
Bromination
48c1dcf50945076da40bbd7976060ec1ea74b3478ef8c25d67664232b218095c
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
c1ccccc1
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#8:2]-[c:3](:[c:4]):[cH;D2;+0:5]:[c:6]:[c:7]-[C:8]=[O;D1;H0:9]>>[#8:2]-[c:3](:[c:4]):[c;H0;D3;+0:5](-[Br;H0;D1;+0:1]):[c:6]:[c:7]-[C:8]=[O;D1;H0:9]
62.6
[{"value": 62.0, "product": "BrC=1C=C(C=O)C=CC1OC(F)(F)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 62.6, "product": "BrC=1C=C(C=O)C=CC1OC(F)(F)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
4
DAY
To a solution of 4-trifluoromethoxybenzaldehyde (215.0 g, 1.13 mol) in a mixture of TFA (300 mL), CH2Cl2 (300 mL) and H2SO4 (150 mL) was added at room temperature N-bromosuccinimide (402.0 g, 2.26 mol) in equal portions over seven hours. The reaction mixture was stirred for four days at room temperature, poured into ic...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
C1CCNC1.c1ccccc1
c1ccccc1
c1ccccc1
HO-
C(=O)(C(F)(F)F)O
null
96
O=C1CCC(=O)N1Br.O=Cc1ccc(OC(F)(F)F)cc1>C(=O)(C(F)(F)F)O>O=Cc1ccc(OC(F)(F)F)c(Br)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ead6c7a55c0f45819004235a7a0643e8
Cc1cc2c(cc1B(O)O)C(C)(C)CCC2(C)C.O=Cc1ccc(OC(F)(F)F)c(Br)c1>>Cc1cc2c(cc1-c1ccc(C=O)cc1OC(F)(F)F)C(C)(C)CCC2(C)C
C([O-])([O-])=O.[K+].[K+].BrC=1C=C(C=O)C=CC1OC(F)(F)F.CC=1C(=CC=2C(CCC(C2C1)(C)C)(C)C)B(O)O.C(C)O>>FC(OC=1C=C(C=O)C=CC1C1=CC=2C(CCC(C2C=C1C)(C)C)(C)C)(F)F
OB(O)[c:7]1[c:2]([CH3:1])[cH:3][c:4]2[c:5]([cH:6]1)[C:21]([CH3:22])([CH3:23])[CH2:24][CH2:25][C:26]2([CH3:27])[CH3:28].Br[c:15]1[c:8]([O:16][C:17]([F:18])([F:19])[F:20])[cH:9][cH:10][c:11]([CH:12]=[O:13])[cH:14]1>>[CH3:1][c:2]1[cH:3][c:4]2[c:5]([cH:6][c:7]1-[c:8]1[cH:9][cH:10][c:11]([CH:12]=[O:13])[cH:14][c:15]1[O:16][...
Cc1cc2c(cc1B(O)O)C(C)(C)CCC2(C)C.O=Cc1ccc(OC(F)(F)F)c(Br)c1
Cc1cc2c(cc1-c1ccc(C=O)cc1OC(F)(F)F)C(C)(C)CCC2(C)C
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.C1(=CC=CC=C1)C.C(C)(=O)OCC
Heteroatom Alkylation and Arylation
OtherReaction
7dac6989769981bfec04459edc6c09b6186b097cedd6dde9f0515c1cc3b2b79c
5a6d5feecbca47ed9520143f4e9a586cd17e903950cdaedb0666222ddfc9f2ae
c1ccc(-c2ccc3c(c2)CCCC3)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[C:4]=[O;D1;H0:5]):[c:6]:[c:7]:[c;H0;D3;+0:8]:1-[O;H0;D2;+0:9]-[C:10](-[F;D1;H0:11])(-[F;D1;H0:12])-[F;D1;H0:13].O-B(-O)-[c;H0;D3;+0:14](:[c:15]:[c:16]):[c:17](-[C;D1;H3:18]):[c:19]>>[C;D1;H3:18]-[c:17](:[c:19]):[c;H0;D3;+0:14](-[c;H0;D3;+0:8]1:[c:7]:[c:6]:[c:3](-[C:4]=[O;D1;H0:5]):[c:2]...
76
[{"value": 76.0, "product": "FC(OC=1C=C(C=O)C=CC1C1=CC=2C(CCC(C2C=C1C)(C)C)(C)C)(F)F", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of 3-bromo-4-trifluoromethoxybenzaldehyde (10.0 g, 37.2 mmol), (3,5,5,8,8-pentamethyl-5,6,7,8-tetrahydronaphthalen-2-yl) boronic acid (11.0 g, 44.68 mmol, 1.2 eq) in a mixture of toluene (100 mL), ethanol (20 mL) and water (15 mL) was added potassium carbonate (10.28 g, 74.4 mmol, 2 eq). The mixture was d...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ether.Boronic acid
Ether
c1ccc2c(c1)CCCC2.c1ccccc1
c1ccccc1.c1ccc2c(c1)CCCC2
c1ccccc1.c1ccc2c(c1)CCCC2
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.C1(=CC=CC=C1)C.C(C)(=O)OCC
null
null
Cc1cc2c(cc1B(O)O)C(C)(C)CCC2(C)C.O=Cc1ccc(OC(F)(F)F)c(Br)c1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.C1(=CC=CC=C1)C.C(C)(=O)OCC>Cc1cc2c(cc1-c1ccc(C=O)cc1OC(F)(F)F)C(C)(C)CCC2(C)C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-dbc2472a465a4e44abf3015595afaaa0
BrBr.COc1ccccn1>>COc1ccc(Br)cn1
[OH-].[Na+].COC1=NC=CC=C1.C(C)(=O)[O-].[Na+].BrBr>>BrC=1C=CC(=NC1)OC
Br[Br:7].[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][cH:8][n:9]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([Br:7])[cH:8][n:9]1
BrBr.COc1ccccn1
COc1ccc(Br)cn1
null
null
O.C(C)(=O)O
Functional Group Interconversion
Bromination
66a492ff31bfcbb52d9a760416ba269a4cf5a439a6c2ca9c2c3a3ed0a750b974
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1ccncc1
Br-[Br;H0;D1;+0:1].[#7;a:2]1:[c:3]:[c:4]:[c:5]:[cH;D2;+0:6]:[c:7]:1>>[Br;H0;D1;+0:1]-[c;H0;D3;+0:6]1:[c:5]:[c:4]:[c:3]:[#7;a:2]:[c:7]:1
51.3
[{"value": 51.3, "product": "BrC=1C=CC(=NC1)OC", "details": "PERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
To a suspension of 2-methoxypyridine (10.00 g, 0.09 mol) and sodium acetate (8.27 g, 0.10 mmol) in 30 mL of glacial acetic acid was added a solution of bromine in 20 mL glacial acetic acid while maintaining the reaction temperature below 50° C. After 3 hours, 100 mL of H2O was added and the resulting solution neutraliz...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccncc1
c1ccncc1
c1ccncc1
HBr
O.C(C)(=O)O
null
3
BrBr.COc1ccccn1>O.C(C)(=O)O>COc1ccc(Br)cn1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5b4a3d696a6b428ba74a62ddda05b982
COc1ccc(C=O)cc1-c1cc2c(cc1C)C(C)(C)CCC2(C)C.O=C1CSC(=O)N1CCc1ccccn1>>COc1ccc(C=C2SC(=O)N(CCc3ccccn3)C2=O)cc1-c1cc2c(cc1C)C(C)(C)CCC2(C)C
COC1=C(C=C(C=O)C=C1)C1=CC=2C(CCC(C2C=C1C)(C)C)(C)C.N1=C(C=CC=C1)CCN1C(SCC1=O)=O>>COC1=C(C=C(C=C2C(N(C(S2)=O)CCC2=NC=CC=C2)=O)C=C1)C1=CC=2C(CCC(C2C=C1C)(C)C)(C)C
O=[CH:7][c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[c:24](-[c:25]2[cH:26][c:27]3[c:28]([cH:29][c:30]2[CH3:31])[C:32]([CH3:33])([CH3:34])[CH2:35][CH2:36][C:37]3([CH3:38])[CH3:39])[cH:23]1.[CH2:8]1[S:9][C:10](=[O:11])[N:12]([CH2:13][CH2:14][c:15]2[cH:16][cH:17][cH:18][cH:19][n:20]2)[C:21]1=[O:22]>>[CH3:1][O:2][c:3]1[cH:4][cH:5...
COc1ccc(C=O)cc1-c1cc2c(cc1C)C(C)(C)CCC2(C)C.O=C1CSC(=O)N1CCc1ccccn1
COc1ccc(C=C2SC(=O)N(CCc3ccccn3)C2=O)cc1-c1cc2c(cc1C)C(C)(C)CCC2(C)C
null
null
null
C-C Coupling
Aldol condensation
315c5abda6f5c04d5321614cd32fbf107303aab42297b04d1819d58208c94487
d1104e4dc387c28c5ac408eab23aa043e968d3cfd16e99022454bf87ce31f401
O=C1SC(=Cc2cccc(-c3ccc4c(c3)CCCC4)c2)C(=O)N1CCc1ccccn1
O=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4].[C:5]-[#7:6]1-[C:7](=[O;D1;H0:8])-[#16:9]-[CH2;D2;+0:10]-[C:11]-1=[O;D1;H0:12]>>[C:5]-[#7:6]1-[C:7](=[O;D1;H0:8])-[#16:9]-[C;H0;D3;+0:10](=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4])-[C:11]-1=[O;D1;H0:12]
null
[]
null
null
null
null
5-[4-Methoxy-3-(3,5,5,8,8-pentamethyl-5,6,7,8-tetrahydro-naphthalen-2-yl)-benzylidene]-3-(2-pyridin-2-yl-ethyl)-thiazolidine-2,4-dione was prepared in a similar manner as described in Example 1 using 4-methoxy-3-(3,5,5,8,8-pentamethyl-5,6,7,8-tetrahydro-naphthalen-2-yl) benzaldehyde and 3-(2-pyridin-2-yl-ethyl)-thiazol...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Monosulfide
Monosulfide
C1CSC[NH]1
C1CSC[NH]1
c1ccccc1.C1CSC[NH]1.c1ccncc1.c1ccc2c(c1)CCCC2
HO-
null
null
null
COc1ccc(C=O)cc1-c1cc2c(cc1C)C(C)(C)CCC2(C)C.O=C1CSC(=O)N1CCc1ccccn1>>COc1ccc(C=C2SC(=O)N(CCc3ccccn3)C2=O)cc1-c1cc2c(cc1C)C(C)(C)CCC2(C)C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-8369fb21e4244d40930a6dee8735a0a3
CN(C)c1cc2c(cc1C=O)C(C)(C)CCC2(C)C.O=C(O)CN1C(=O)CSC1=S>>CN(C)c1cc2c(cc1-c1ccc3cc(C=C4SC(=S)N(CC(=O)O)C4=O)ccc3c1)C(C)(C)CCC2(C)C
CN(C=1C(=CC=2C(CCC(C2C1)(C)C)(C)C)C=O)C.S1C(=S)N(C(=O)C1)CC(=O)O>>CN(C=1C(=CC=2C(CCC(C2C1)(C)C)(C)C)C=1C=C2C=CC(=CC2=CC1)C=C1C(N(C(S1)=S)CC(=O)O)=O)C
O=[CH:10][c:9]1[c:4]([N:2]([CH3:1])[CH3:3])[cH:5][c:6]2[c:7]([cH:8]1)[C:32]([CH3:33])([CH3:34])[CH2:35][CH2:36][C:37]2([CH3:11])[CH3:12].[CH2:17]1[S:18][C:19](=[S:20])[N:21]([CH2:22][C:23](=[O:24])[OH:25])[C:26]1=[O:27]>>[CH3:1][N:2]([CH3:3])[c:4]1[cH:5][c:6]2[c:7]([cH:8][c:9]1-[c:10]1[cH:11][cH:12][c:13]3[cH:14][c:15]...
CN(C)c1cc2c(cc1C=O)C(C)(C)CCC2(C)C.O=C(O)CN1C(=O)CSC1=S
CN(C)c1cc2c(cc1-c1ccc3cc(C=C4SC(=S)N(CC(=O)O)C4=O)ccc3c1)C(C)(C)CCC2(C)C
null
null
null
C-C Coupling
OtherReaction
e8323e93057d9dc5b72df472f79adc1b56d688c7074d60002ae7aab28e700d6b
d1104e4dc387c28c5ac408eab23aa043e968d3cfd16e99022454bf87ce31f401
O=C1NC(=S)SC1=Cc1ccc2cc(-c3ccc4c(c3)CCCC4)ccc2c1
O=[CH;D2;+0:1]-[c;H0;D3;+0:2]1:[c:3]:[c:4]:[c:5](:[c:6]:[c:7]:1-[#7:8])-[C;H0;D4;+0:9](-[CH3;D1;+0:10])(-[CH3;D1;+0:11])-[C:12]-[C:13].[O;D1;H0:14]=[C:15](-[O;D1;H1:16])-[C:17]-[#7:18]1-[C:19](=[S;D1;H0:20])-[#16:21]-[CH2;D2;+0:22]-[C:23]-1=[O;D1;H0:24]>>[#7:8]-[c:7]1:[c:6]:[c:5](:[c:4]:[c:3]:[c;H0;D3;+0:2]:1-[c;H0;D3;...
null
[]
null
null
null
null
{5-[6-(3-Dimethylamino-5,5,8,8-tetramethyl-5,6,7,8-tetrahydro-naphthalen-2-yl)-naphthalen-2-yl methylene]-4-oxo-2-thioxo-thiazolidin-3-yl}-acetic acid was prepared in a similar manner as described in Example 1 using 6-(3-dimethylamino-5,5,8,8-tetramethyl-5,6,7,8-tetrahydro-naphthalen-2-carboxaldehyde and rhodanine acet...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Monosulfide
Monosulfide
c1ccc2c(c1)CCCC2.C1CSC[NH]1
c1ccc2ccccc2c1.C1CSC[NH]1.c1ccc2c(c1)CCCC2
c1ccc2ccccc2c1.C1CSC[NH]1.c1ccc2c(c1)CCCC2
null
null
null
null
CN(C)c1cc2c(cc1C=O)C(C)(C)CCC2(C)C.O=C(O)CN1C(=O)CSC1=S>>CN(C)c1cc2c(cc1-c1ccc3cc(C=C4SC(=S)N(CC(=O)O)C4=O)ccc3c1)C(C)(C)CCC2(C)C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5f1461830198416ea9317c089d13033f
CCO.O=C(O)c1ccc2cc(O)ccc2c1>>CCOC(=O)c1ccc2cc(O)ccc2c1
OC=1C=C2C=CC(=CC2=CC1)C(=O)O.C(C)O>>C(C)OC(=O)C1=CC2=CC=C(C=C2C=C1)O
[CH3:1][CH2:2][OH:3].O[C:4](=[O:5])[c:6]1[cH:7][cH:8][c:9]2[cH:10][c:11]([OH:12])[cH:13][cH:14][c:15]2[cH:16]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][c:9]2[cH:10][c:11]([OH:12])[cH:13][cH:14][c:15]2[cH:16]1
CCO.O=C(O)c1ccc2cc(O)ccc2c1
CCOC(=O)c1ccc2cc(O)ccc2c1
null
null
S(O)(O)(=O)=O
Protection
Esterification of Carboxylic Acids
070670f68a20c1021da94fabee54def4688122fb721af5f52cd5a03630845d0e
0d8a72b7375d91aa7263e766e03a3cb7c4fa91e27abcd590409ff03b98eed690
c1ccc2ccccc2c1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C;D1;H3:6]-[C:7]-[OH;D1;+0:8]>>[C;D1;H3:6]-[C:7]-[O;H0;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
null
[]
null
null
16
HOUR
A solution of 6-hydroxy-2-naphthoic acid (75.9 g, 0.40 mol) in ethanol (1.0 L) and sulfuric acid (5.0 mL) was heated to reflux under an atmosphere of nitrogen. After 16 hours, the volume was removed to approximately half via simple distillation and the resulting solution was diluted with water. The resulting cloudy mix...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary alcohol
Ester
null
null
c1ccc2ccccc2c1
HO-
S(O)(O)(=O)=O
null
16
CCO.O=C(O)c1ccc2cc(O)ccc2c1>S(O)(O)(=O)=O>CCOC(=O)c1ccc2cc(O)ccc2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b6cb880dfda64425bb78ed2cb9037e1b
CCOC(=O)c1ccc2cc(OS(=O)(=O)C(F)(F)F)ccc2c1>>O=S(=O)(Oc1ccc2cc(CO)ccc2c1)C(F)(F)F
C(C)OC(=O)C1=CC2=CC=C(C=C2C=C1)OS(=O)(=O)C(F)(F)F.CC(C)C[AlH]CC(C)C>>FC(S(=O)(=O)OC=1C=C2C=CC(=CC2=CC1)CO)(F)F
CCO[C:11]([c:10]1[cH:9][c:8]2[cH:7][cH:6][c:5]([O:4][S:2](=[O:1])(=[O:3])[C:17]([F:18])([F:19])[F:20])[cH:16][c:15]2[cH:14][cH:13]1)=[O:12]>>[O:1]=[S:2](=[O:3])([O:4][c:5]1[cH:6][cH:7][c:8]2[cH:9][c:10]([CH2:11][OH:12])[cH:13][cH:14][c:15]2[cH:16]1)[C:17]([F:18])([F:19])[F:20]
CCOC(=O)c1ccc2cc(OS(=O)(=O)C(F)(F)F)ccc2c1
O=S(=O)(Oc1ccc2cc(CO)ccc2c1)C(F)(F)F
null
null
C1(=CC=CC=C1)C
Functional Group Interconversion
Reduction of ester to primary alcohol
cd99347e3144bc4f081bc664a4bc5a11d1e392f7cea47a5adad92bcd498ccf56
a2b5cf843cfeb048c76ac4cbf0bd8ccab026fcad80259b78e012cdb6ac2f5934
c1ccc2ccccc2c1
C-C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3](:[c:4]):[c:5]>>[OH;D1;+0:2]-[CH2;D2;+0:1]-[c:3](:[c:4]):[c:5]
72
[{"value": 72.0, "product": "FC(S(=O)(=O)OC=1C=C2C=CC(=CC2=CC1)CO)(F)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 71.6, "product": "FC(S(=O)(=O)OC=1C=C2C=CC(=CC2=CC1)CO)(F)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a slurry of 6-trifluoromethanesulfonyloxy-naphthalene-2-carboxylic acid ethyl ester (136.50 g, 0.392 mol) in toluene (1.0 L) at −70° C. was added a solution of DIBAL (1.5 M, 5.75 mL, 0.862 mol) dropwise while maintaining an internal temperature below −55° C. The resulting mixture was allowed to stir for 1 hour and s...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
c1ccc2ccccc2c1
HO-
C1(=CC=CC=C1)C
null
1
CCOC(=O)c1ccc2cc(OS(=O)(=O)C(F)(F)F)ccc2c1>C1(=CC=CC=C1)C>O=S(=O)(Oc1ccc2cc(CO)ccc2c1)C(F)(F)F
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-69ef83815cd34e009ed65d285bc956f6
O=S(=O)(Oc1ccc2cc(CO)ccc2c1)C(F)(F)F>>O=Cc1ccc2cc(OS(=O)(=O)C(F)(F)F)ccc2c1
FC(S(=O)(=O)OC=1C=C2C=CC(=CC2=CC1)CO)(F)F.C=1C=C[NH+]=CC1.[O-][Cr](=O)(=O)Cl>>FC(S(=O)(=O)OC=1C=C2C=CC(=CC2=CC1)C=O)(F)F
[OH:1][CH2:2][c:3]1[cH:4][cH:5][c:6]2[cH:7][c:8]([O:9][S:10](=[O:11])(=[O:12])[C:13]([F:14])([F:15])[F:16])[cH:17][cH:18][c:19]2[cH:20]1>>[O:1]=[CH:2][c:3]1[cH:4][cH:5][c:6]2[cH:7][c:8]([O:9][S:10](=[O:11])(=[O:12])[C:13]([F:14])([F:15])[F:16])[cH:17][cH:18][c:19]2[cH:20]1
O=S(=O)(Oc1ccc2cc(CO)ccc2c1)C(F)(F)F
O=Cc1ccc2cc(OS(=O)(=O)C(F)(F)F)ccc2c1
null
null
C(Cl)Cl
Oxidation
Oxidation or Dehydrogenation of Alcohols to Aldehydes and Ketones
41bfa9deea81b465c88ad21fdfb64a2e1ba29490558cf430df132cb98b4a538b
0a03c6724c1862e8f86d4a463afda55b8e067dc6cb42597b472eb7cabc03eda3
c1ccc2ccccc2c1
[OH;D1;+0:1]-[CH2;D2;+0:2]-[c:3](:[c:4]):[c:5]>>[O;H0;D1;+0:1]=[CH;D2;+0:2]-[c:3](:[c:4]):[c:5]
94
[{"value": 94.0, "product": "FC(S(=O)(=O)OC=1C=C2C=CC(=CC2=CC1)C=O)(F)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 93.8, "product": "FC(S(=O)(=O)OC=1C=C2C=CC(=CC2=CC1)C=O)(F)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a mechanical stirred solution of 6-trifluoromethanesulfonyloxy-naphthalen-2-yl-methanol (70.0 g, 0.228 mol) in CH2Cl2 (600 mL) under an atmosphere of argon was added PCC (54.20 g, 0.25 mol, crushed prior to addition) over a few minutes. After 2 hours the resulting black suspension was poured onto a silica gel column...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Aldehyde
null
null
c1ccc2ccccc2c1
null
C(Cl)Cl
null
null
O=S(=O)(Oc1ccc2cc(CO)ccc2c1)C(F)(F)F>C(Cl)Cl>O=Cc1ccc2cc(OS(=O)(=O)C(F)(F)F)ccc2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c298b3b7776043f6998b7e42bc24f8c8
CC1(C)CCC(C)(C)c2cc([N+](=O)[O-])ccc21>>CC1(C)CCC(C)(C)c2cc(N)ccc21
[N+](=O)([O-])C1=CC=2C(CCC(C2C=C1)(C)C)(C)C.[H][H]>>NC1=CC=2C(CCC(C2C=C1)(C)C)(C)C
O=[N+:12]([O-])[c:11]1[cH:10][c:9]2[c:15]([cH:14][cH:13]1)[C:2]([CH3:1])([CH3:3])[CH2:4][CH2:5][C:6]2([CH3:7])[CH3:8]>>[CH3:1][C:2]1([CH3:3])[CH2:4][CH2:5][C:6]([CH3:7])([CH3:8])[c:9]2[cH:10][c:11]([NH2:12])[cH:13][cH:14][c:15]21
CC1(C)CCC(C)(C)c2cc([N+](=O)[O-])ccc21
CC1(C)CCC(C)(C)c2cc(N)ccc21
null
[Pd]
ClCCl
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc2c(c1)CCCC2
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
To a solution of 2-nitro-5,5,8,8-tetramethyl-5,6,7,8-tetrahydro-naphthalene (79.0 g, 0.339 mol) in dichloromethane as added 1 g of 10% palladium on carbon and the mixture was hydrogenated at 40–50 psi of hydrogen for 20 hrs. The catalyst was removed by filtration and the organic and the aqueous layers were separated. T...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccc2c(c1)CCCC2
Other
[Pd].ClCCl
null
null
CC1(C)CCC(C)(C)c2cc([N+](=O)[O-])ccc21>[Pd].ClCCl>CC1(C)CCC(C)(C)c2cc(N)ccc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-8c3f080bf557442fbfb92d96788e8437
C=O.CC1(C)CCC(C)(C)c2cc(N)ccc21>>CN(C)c1ccc2c(c1)C(C)(C)CCC2(C)C
C(C)(=O)O.NC1=CC=2C(CCC(C2C=C1)(C)C)(C)C.C=O.C(#N)[BH3-].[Na+]>>CN(C1=CC=2C(CCC(C2C=C1)(C)C)(C)C)C
O=[CH2:3].[NH2:2][c:4]1[cH:5][cH:6][c:7]2[c:8]([cH:9]1)[C:10]([CH3:11])([CH3:12])[CH2:13][CH2:14][C:15]2([CH3:16])[CH3:17]>>[CH3:1][N:2]([CH3:3])[c:4]1[cH:5][cH:6][c:7]2[c:8]([cH:9]1)[C:10]([CH3:11])([CH3:12])[CH2:13][CH2:14][C:15]2([CH3:16])[CH3:17]
C=O.CC1(C)CCC(C)(C)c2cc(N)ccc21
CN(C)c1ccc2c(c1)C(C)(C)CCC2(C)C
null
null
C(C)#N
Heteroatom Alkylation and Arylation
Eschweiler-Clarke Primary Amine Methylation
5bc40be4d4b4346801fbfcec480fec37de3ff2eecebe2990b3686fa4792d12b6
5cdbf447f632627824e84e0bcac2293ea9ebd70c19b0d56dea90691653b444c7
c1ccc2c(c1)CCCC2
O=[CH2;D1;+0:1].[NH2;D1;+0:2]-[c:3](:[c:4]):[c:5]>>[C;D1;H3:6]-[N;H0;D3;+0:2](-[CH3;D1;+0:1])-[c:3](:[c:4]):[c:5]
70
[{"value": 70.0, "product": "CN(C1=CC=2C(CCC(C2C=C1)(C)C)(C)C)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
To a solution of 2-amino-5,5,8,8-tetramethyl-5,6,7,8-tetrahydronaphthalene (70.10 g, 0.345 mol) and formaldehyde (280 mL, 10 eq) in 2 L of acetonitrile cooled to 0° C. was added sodium cyanoborohydride (65 g, 3 eq.) in portions while maintaining the temperature between 10–20° C. Glacial acetic acid was added to adjust ...
10.6084/m9.figshare.5104873.v1
null
Formaldehyde.Primary amine
Tertiary amine
null
null
c1ccc2c(c1)CCCC2
null
C(C)#N
null
2
C=O.CC1(C)CCC(C)(C)c2cc(N)ccc21>C(C)#N>CN(C)c1ccc2c(c1)C(C)(C)CCC2(C)C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a1901d57fac948e9a496e91086c3a4e7
CC(C)OB(OC(C)C)OC(C)C.CN(C)c1cc2c(cc1Br)C(C)(C)CCC2(C)C>>CN(C)c1cc2c(cc1B(O)O)C(C)(C)CCC2(C)C
B(OC(C)C)(OC(C)C)OC(C)C.BrC1=CC=2C(CCC(C2C=C1N(C)C)(C)C)(C)C.C(CCC)[Li].Cl>>CN(C=1C(=CC=2C(CCC(C2C1)(C)C)(C)C)B(O)O)C
CC(C)O[B:10]([O:11]C(C)C)[O:12]C(C)C.Br[c:9]1[c:4]([N:2]([CH3:1])[CH3:3])[cH:5][c:6]2[c:7]([cH:8]1)[C:13]([CH3:14])([CH3:15])[CH2:16][CH2:17][C:18]2([CH3:19])[CH3:20]>>[CH3:1][N:2]([CH3:3])[c:4]1[cH:5][c:6]2[c:7]([cH:8][c:9]1[B:10]([OH:11])[OH:12])[C:13]([CH3:14])([CH3:15])[CH2:16][CH2:17][C:18]2([CH3:19])[CH3:20]
CC(C)OB(OC(C)C)OC(C)C.CN(C)c1cc2c(cc1Br)C(C)(C)CCC2(C)C
CN(C)c1cc2c(cc1B(O)O)C(C)(C)CCC2(C)C
null
null
C1CCOC1
Miscellaneous
Preparation of boronic acids
44976aedc627652e57cf654966855ab06a9db6d01924d4ea2bf9f8b5ec0f6db6
dafd25fbe01879c365f8c874026e570f49824f4bb82016b29d0c5d21aeb58ca3
c1ccc2c(c1)CCCC2
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[#7:5]):[c:6].C-C(-C)-O-[B;H0;D3;+0:7](-[O;H0;D2;+0:8]-C(-C)-C)-[O;H0;D2;+0:9]-C(-C)-C>>[#7:5]-[c:4](:[c:6]):[c;H0;D3;+0:1](-[B;H0;D3;+0:7](-[OH;D1;+0:8])-[OH;D1;+0:9]):[c:2]:[c:3]
39
[{"value": 39.0, "product": "CN(C=1C(=CC=2C(CCC(C2C1)(C)C)(C)C)B(O)O)C", "details": "PERCENTYIELD", "is_desired": false}]
-78
CELSIUS
10
MINUTE
To a solution of 2-Bromo-3-dimethylamino-5,5,8,8-tetramethyl-5,6,7,8-tetrahydronaphthalene (67.08 g, 0.216 mol) in 300 mL of anhydrous THF at −78° C. was added dropwise at −78° C. a 1.6 molar solution of n-butyl lithium (1.6 M, 203 mL, 1.5 eq.) over a period of 30 minutes. The reaction was stirred for 10 min. at −78° C...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
Boronic acid
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2
HBr
C1CCOC1
-78
0.166667
CC(C)OB(OC(C)C)OC(C)C.CN(C)c1cc2c(cc1Br)C(C)(C)CCC2(C)C>C1CCOC1>CN(C)c1cc2c(cc1B(O)O)C(C)(C)CCC2(C)C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ecb4f7b1ddfc45b2a209c0bd72c64a72
CN(C)c1ccc(C=O)cc1.[Br-]>>CN(C)c1ccc(C=O)cc1Br
CN(C1=CC=C(C=O)C=C1)C.[Br-].[Br-].[Br-].[NH+]1=CC=CC=C1.[NH+]1=CC=CC=C1.[NH+]1=CC=CC=C1>>BrC=1C=C(C=O)C=CC1N(C)C
[CH3:1][N:2]([CH3:3])[c:4]1[cH:5][cH:6][c:7]([CH:8]=[O:9])[cH:10][cH:11]1.[Br-:12]>>[CH3:1][N:2]([CH3:3])[c:4]1[cH:5][cH:6][c:7]([CH:8]=[O:9])[cH:10][c:11]1[Br:12]
CN(C)c1ccc(C=O)cc1.[Br-]
CN(C)c1ccc(C=O)cc1Br
null
null
ClCCl
Functional Group Interconversion
Bromination
f6effe61353895b318215d8bd9b6bb1105cafbf7be8c217d748df587260b32c3
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1ccccc1
[#7:1]-[c:2](:[c:3]):[cH;D2;+0:4]:[c:5]:[c:6]-[C:7]=[O;D1;H0:8].[Br-;H0;D0:9]>>[#7:1]-[c:2](:[c:3]):[c;H0;D3;+0:4](-[Br;H0;D1;+0:9]):[c:5]:[c:6]-[C:7]=[O;D1;H0:8]
92
[{"value": 92.0, "product": "BrC=1C=C(C=O)C=CC1N(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 92.0, "product": "BrC=1C=C(C=O)C=CC1N(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To a solution of 4-(dimethylamino)-benzaldehyde (10.0 g, 67.03 mmol) in dichloromethane (250 mL) was added pyridinium tribromide (21.4 g, 67.03 mmol). The reaction mixture was stirred at room temperature overnight. The solution was washed successively with water and brine, dried over anhydrous magnesium sulfate, filter...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccccc1
c1ccccc1
c1ccccc1
null
ClCCl
null
8
CN(C)c1ccc(C=O)cc1.[Br-]>ClCCl>CN(C)c1ccc(C=O)cc1Br
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5b00ee9768ad48a898dd923a0cb62874
CN1C(=O)CSC1=O.Cc1cc2c(cc1-c1cc(C=O)ccc1OC(F)(F)F)N(C)C(=O)CC2(C)C>>Cc1cc2c(cc1-c1cc(C=C3SC(=O)N(C)C3=O)ccc1OC(F)(F)F)N(C)C(=O)CC2(C)C
C1(=CC=CC=C1)C.N1CCCCC1.CN1C(CC(C2=CC(=C(C=C12)C=1C=C(C=O)C=CC1OC(F)(F)F)C)(C)C)=O.CN1C(SCC1=O)=O>>CN1C(SC(C1=O)=CC1=CC(=C(C=C1)OC(F)(F)F)C1=C(C=C2C(CC(N(C2=C1)C)=O)(C)C)C)=O
[CH2:12]1[S:13][C:14](=[O:15])[N:16]([CH3:17])[C:18]1=[O:19].O=[CH:11][c:10]1[cH:9][c:8](-[c:7]2[c:2]([CH3:1])[cH:3][c:4]3[c:5]([cH:6]2)[N:28]([CH3:29])[C:30](=[O:31])[CH2:32][C:33]3([CH3:34])[CH3:35])[c:22]([O:23][C:24]([F:25])([F:26])[F:27])[cH:21][cH:20]1>>[CH3:1][c:2]1[cH:3][c:4]2[c:5]([cH:6][c:7]1-[c:8]1[cH:9][c:1...
CN1C(=O)CSC1=O.Cc1cc2c(cc1-c1cc(C=O)ccc1OC(F)(F)F)N(C)C(=O)CC2(C)C
Cc1cc2c(cc1-c1cc(C=C3SC(=O)N(C)C3=O)ccc1OC(F)(F)F)N(C)C(=O)CC2(C)C
null
null
C(C)(=O)O.C(C)(=O)OCC
C-C Coupling
Aldol condensation
315c5abda6f5c04d5321614cd32fbf107303aab42297b04d1819d58208c94487
d1104e4dc387c28c5ac408eab23aa043e968d3cfd16e99022454bf87ce31f401
O=C1CCc2ccc(-c3cccc(C=C4SC(=O)NC4=O)c3)cc2N1
O=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4].[C;D1;H3:5]-[#7:6]1-[C:7](=[O;D1;H0:8])-[#16:9]-[CH2;D2;+0:10]-[C:11]-1=[O;D1;H0:12]>>[C;D1;H3:5]-[#7:6]1-[C:7](=[O;D1;H0:8])-[#16:9]-[C;H0;D3;+0:10](=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4])-[C:11]-1=[O;D1;H0:12]
null
[]
null
null
null
null
A mixture of toluene (80 mL), piperidine (380 μL), acetic acid (380 μL), 3-(1,4,4,6-Tetramethyl-2-oxo-1,2,3,4-tetrahydro-quinolin-7-yl)-4-trifluoromethoxy-benzaldehyde (7.5 g, 19.16 mmol) and a 3-alkyl—thiazolidine-2,4-dione such as 3-Methyl-thiazolidine-2,4-dione (19.16 mmol) is heated at reflux overnight. The reactio...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Monosulfide
Monosulfide
C1CSC[NH]1
C1CSC[NH]1
c1ccccc1.C1CSC[NH]1.c1ccc2c(c1)CCC[NH]2
HO-
C(C)(=O)O.C(C)(=O)OCC
null
null
CN1C(=O)CSC1=O.Cc1cc2c(cc1-c1cc(C=O)ccc1OC(F)(F)F)N(C)C(=O)CC2(C)C>C(C)(=O)O.C(C)(=O)OCC>Cc1cc2c(cc1-c1cc(C=C3SC(=O)N(C)C3=O)ccc1OC(F)(F)F)N(C)C(=O)CC2(C)C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4b65c66c2fa4497087cd2562941f4a17
CI.Cc1cc2c(cc1Br)NC(=O)CC2(C)C>>Cc1cc2c(cc1Br)N(C)C(=O)CC2(C)C
O.BrC1=C(C=C2C(CC(NC2=C1)=O)(C)C)C.[OH-].[K+].CI>>BrC1=C(C=C2C(CC(N(C2=C1)C)=O)(C)C)C
I[CH3:10].[CH3:1][c:2]1[cH:3][c:4]2[c:5]([cH:6][c:7]1[Br:8])[NH:9][C:11](=[O:12])[CH2:13][C:14]2([CH3:15])[CH3:16]>>[CH3:1][c:2]1[cH:3][c:4]2[c:5]([cH:6][c:7]1[Br:8])[N:9]([CH3:10])[C:11](=[O:12])[CH2:13][C:14]2([CH3:15])[CH3:16]
CI.Cc1cc2c(cc1Br)NC(=O)CC2(C)C
Cc1cc2c(cc1Br)N(C)C(=O)CC2(C)C
null
null
CS(=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
28e9bbae9e351621b70430e528cb53ce2fca2ea13e7a82f3ed5f3b0a20d55e94
0a16658309ac5595448433dd7ef49294830b145345df0b202ccd54727262e629
O=C1CCc2ccccc2N1
I-[CH3;D1;+0:1].[C:2]-[C:3](=[O;D1;H0:4])-[NH;D2;+0:5]-[c:6](:[c:7]):[c:8]>>[C:2]-[C:3](=[O;D1;H0:4])-[N;H0;D3;+0:5](-[CH3;D1;+0:1])-[c:6](:[c:7]):[c:8]
101.3
[{"value": 99.0, "product": "BrC1=C(C=C2C(CC(N(C2=C1)C)=O)(C)C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 101.3, "product": "BrC1=C(C=C2C(CC(N(C2=C1)C)=O)(C)C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
10
MINUTE
A mixture of powdered KOH (14.06 g, 0.250 mol) in DMSO (150 mL) was stirred at 0° C. for 10 min. 7-Bromo-4,4,6-trimethyl-3,4-dihydro-1H-quinoline-2-one (33.59 g, 0.125 mol) was added cautiously, followed immediately by the addition of methyl iodide (39 mL, 0.625 mol). The reaction mixture was kept at 0° C. for 30 min t...
10.6084/m9.figshare.5104873.v1
null
Secondary amide
Tertiary amide
c1ccc2c(c1)CCCN2
c1ccc2c(c1)CCC[NH]2
c1ccc2c(c1)CCC[NH]2
HI
CS(=O)C
0
0.166667
CI.Cc1cc2c(cc1Br)NC(=O)CC2(C)C>CS(=O)C>Cc1cc2c(cc1Br)N(C)C(=O)CC2(C)C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-dbf0f186371046a78ad1fca5bc79a0a1
CC(C)=CC(=O)Nc1ccc(C)c(Br)c1>>Cc1cc2c(cc1Br)NC(=O)CC2(C)C
BrC=1C=C(C=CC1C)NC(C=C(C)C)=O.[Cl-].[Al+3].[Cl-].[Cl-]>>BrC1=C(C=C2C(CC(NC2=C1)=O)(C)C)C
[CH3:1][c:2]1[cH:3][cH:4][c:5]([NH:9][C:10](=[O:11])[CH:12]=[C:13]([CH3:14])[CH3:15])[cH:6][c:7]1[Br:8]>>[CH3:1][c:2]1[cH:3][c:4]2[c:5]([cH:6][c:7]1[Br:8])[NH:9][C:10](=[O:11])[CH2:12][C:13]2([CH3:14])[CH3:15]
CC(C)=CC(=O)Nc1ccc(C)c(Br)c1
Cc1cc2c(cc1Br)NC(=O)CC2(C)C
null
null
null
C-C Coupling
OtherReaction
aea010e81c6715af41577808b3395b1a500e0b61256ebfb3a34fc3616fdf9072
410ec9b1cc243569e4ff568c248f0b402403802e002b4018f576af3f6960507b
O=C1CCc2ccccc2N1
[C;D1;H3:1]-[C;H0;D3;+0:2](-[C;D1;H3:3])=[CH;D2;+0:4]-[C:5](=[O;D1;H0:6])-[#7:7]-[c:8](:[c:9]):[cH;D2;+0:10]:[c:11]:[c:12]>>[C;D1;H3:1]-[C;H0;D4;+0:2]1(-[C;D1;H3:3])-[CH2;D2;+0:4]-[C:5](=[O;D1;H0:6])-[#7:7]-[c:8](:[c:9]):[c;H0;D3;+0:10]-1:[c:11]:[c:12]
65.7
[{"value": 65.7, "product": "BrC1=C(C=C2C(CC(NC2=C1)=O)(C)C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
To a solution of 3-methyl-but-2-enoic acid (3-bromo-4-methyl-phenyl)-amide (70.0 g, 261 mmol) at 90° C. was added portion wise, under argon, with vigorous stirring aluminum chloride (52.3 g, 391 mmol) over 1.5 hr. The reaction mixture was stirred for 2 hours at 110–120° C. The reaction mixture was cooled to room temper...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ccccc1
c1ccc2c(c1)CCCN2
c1ccc2c(c1)CCCN2
null
null
null
2
CC(C)=CC(=O)Nc1ccc(C)c(Br)c1>>Cc1cc2c(cc1Br)NC(=O)CC2(C)C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e4616a7bf65640f491ce4b54c4225ed0
CC(C)=CC(=O)Cl.Cc1ccc(N)cc1Br>>CC(C)=CC(=O)Nc1ccc(C)c(Br)c1
BrC=1C=C(N)C=CC1C.[OH-].[Na+].CC(=CC(=O)Cl)C>>BrC=1C=C(C=CC1C)NC(C=C(C)C)=O
Cl[C:5]([CH:4]=[C:2]([CH3:1])[CH3:3])=[O:6].[NH2:7][c:8]1[cH:9][cH:10][c:11]([CH3:12])[c:13]([Br:14])[cH:15]1>>[CH3:1][C:2]([CH3:3])=[CH:4][C:5](=[O:6])[NH:7][c:8]1[cH:9][cH:10][c:11]([CH3:12])[c:13]([Br:14])[cH:15]1
CC(C)=CC(=O)Cl.Cc1ccc(N)cc1Br
CC(C)=CC(=O)Nc1ccc(C)c(Br)c1
null
null
ClCCl.O
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
c1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]=[C:4](-[C;D1;H3:5])-[C;D1;H3:6].[NH2;D1;+0:7]-[c:8](:[c:9]):[c:10]>>[C;D1;H3:5]-[C:4](-[C;D1;H3:6])=[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:7]-[c:8](:[c:9]):[c:10]
97
[{"value": 97.0, "product": "BrC=1C=C(C=CC1C)NC(C=C(C)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 97.0, "product": "BrC=1C=C(C=CC1C)NC(C=C(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
48
HOUR
To a biphasic mixture of 3-bromo-4-methylaniline (50 g, 0.269 mol), 10% NaOH (270 mL) and dichloromethane (160 mL) was added dropwise over a period of 2 hours 3,3-dimethylacryloyl chloride (36 mL, 0.322 mol) in dichloromethane (95 mL). The solution was stirred at room temperature for 48 hours then diluted with water (1...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1ccccc1
HCl
ClCCl.O
null
48
CC(C)=CC(=O)Cl.Cc1ccc(N)cc1Br>ClCCl.O>CC(C)=CC(=O)Nc1ccc(C)c(Br)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c72610874ea448b4a4768ec392bc794b
Cc1ccc([N+](=O)[O-])cc1Br>>Cc1ccc(N)cc1Br
C([O-])([O-])=O.[K+].[K+].BrC1=C(C=CC(=C1)[N+](=O)[O-])C.C(C)O.O.O.[Sn](Cl)Cl>>BrC=1C=C(N)C=CC1C
O=[N+:6]([O-])[c:5]1[cH:4][cH:3][c:2]([CH3:1])[c:8]([Br:9])[cH:7]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([NH2:6])[cH:7][c:8]1[Br:9]
Cc1ccc([N+](=O)[O-])cc1Br
Cc1ccc(N)cc1Br
null
null
C(C)OC(C)=O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccccc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
100
[{"value": 100.0, "product": "BrC=1C=C(N)C=CC1C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To a solution of 2-bromo-4-nitrotoluene (50 g, 0.231 mol in ethylacetate (330 mL) and Ethanol (150 mL) was added Tin(II)chloride dihydrate (208 g, 0.924 mol) portionwise. The reaction mixture was stirred at room temperature overnight. The solution was then treated with potassium carbonate until pH=7 and filtered over c...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1
Other
C(C)OC(C)=O
null
8
Cc1ccc([N+](=O)[O-])cc1Br>C(C)OC(C)=O>Cc1ccc(N)cc1Br
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-77caa91568234d24a077c16a3f1fb4fb
Cc1cc2c(cc1Br)NC(=O)CC2(C)C>>Cc1cc2c(cc1Br)N(C)C(=O)CC2(C)C
O.BrC1=C(C=C2C(CC(NC2=C1)=O)(C)C)C.[OH-].[K+].C(C)I>>BrC1=C(C=C2C(CC(N(C2=C1)C)=O)(C)C)C
[CH3:1][c:2]1[cH:3][c:4]2[c:5]([cH:6][c:7]1[Br:8])[NH:9][C:11](=[O:12])[CH2:13][C:14]2([CH3:15])[CH3:16]>>[CH3:1][c:2]1[cH:3][c:4]2[c:5]([cH:6][c:7]1[Br:8])[N:9]([CH3:10])[C:11](=[O:12])[CH2:13][C:14]2([CH3:15])[CH3:16]
Cc1cc2c(cc1Br)NC(=O)CC2(C)C
Cc1cc2c(cc1Br)N(C)C(=O)CC2(C)C
null
null
CS(=O)C
Miscellaneous
OtherReaction
dfbdcbb9d33b82807e03a0fdd7314a553d6e1569f469cd8b72d4636c9de45108
7fae2ddae661851fbaf2a59d877a8345033038358ec191ec2c5e2351a33f569b
O=C1CCc2ccccc2N1
[C:1]-[C:2](=[O;D1;H0:3])-[NH;D2;+0:4]-[c:5](:[c:6]):[c:7]>>[C:1]-[C:2](=[O;D1;H0:3])-[N;H0;D3;+0:4](-[C;D1;H3:8])-[c:5](:[c:6]):[c:7]
104.5
[{"value": 104.5, "product": "BrC1=C(C=C2C(CC(N(C2=C1)C)=O)(C)C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
10
MINUTE
A mixture of powdered potassium hydroxide (3.35 g, 59.67 mmol) in DMSO (40 mL) was stirred at 0° C. for 10 min. 7-bromo-4,4,6-trimethyl-3,4-dihydro-1H-quinoline-2-one (Example 1e) (8.0 g, 29.83 mmol) was added cautiously, followed immediately by the addition of ethyl iodide (12 mL, 149.17 mmol). The reaction mixture wa...
10.6084/m9.figshare.5104873.v1
null
Secondary amide
Tertiary amide
c1ccc2c(c1)CCCN2
c1ccc2c(c1)CCC[NH]2
c1ccc2c(c1)CCC[NH]2
Other
CS(=O)C
0
0.166667
Cc1cc2c(cc1Br)NC(=O)CC2(C)C>CS(=O)C>Cc1cc2c(cc1Br)N(C)C(=O)CC2(C)C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-976c401de5844f6db056c8abc7fdf8dc
BrBr.Cc1ccc2c(c1)n(C)c(=O)c(=O)n2C>>Cc1cc2c(cc1Br)n(C)c(=O)c(=O)n2C
[OH-].[Na+].O.CN1C(C(N(C2=CC(=CC=C12)C)C)=O)=O.BrBr>>BrC=1C=C2N(C(C(N(C2=CC1C)C)=O)=O)C
Br[Br:8].[CH3:1][c:2]1[cH:3][c:4]2[c:5]([cH:6][cH:7]1)[n:9]([CH3:10])[c:11](=[O:12])[c:13](=[O:14])[n:15]2[CH3:16]>>[CH3:1][c:2]1[cH:3][c:4]2[c:5]([cH:6][c:7]1[Br:8])[n:9]([CH3:10])[c:11](=[O:12])[c:13](=[O:14])[n:15]2[CH3:16]
BrBr.Cc1ccc2c(c1)n(C)c(=O)c(=O)n2C
Cc1cc2c(cc1Br)n(C)c(=O)c(=O)n2C
null
null
C(C)(=O)O
Functional Group Interconversion
Bromination
82e70b0f760eee9ea654cea51b2b5192206b0037c5d0fce055e76049ea3dc1eb
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
O=c1[nH]c2ccccc2[nH]c1=O
Br-[Br;H0;D1;+0:1].[C;D1;H3:2]-[#7;a:3]1:[c:4]:[c:5]:[#7;a:6]:[c:7]2:[c:8]:[c:9](-[C;D1;H3:10]):[cH;D2;+0:11]:[c:12]:[c:13]:1:2>>[Br;H0;D1;+0:1]-[c;H0;D3;+0:11]1:[c:12]:[c:13]2:[#7;a:3](-[C;D1;H3:2]):[c:4]:[c:5]:[#7;a:6]:[c:7]:2:[c:8]:[c:9]:1-[C;D1;H3:10]
99.3
[{"value": 99.3, "product": "BrC=1C=C2N(C(C(N(C2=CC1C)C)=O)=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
50
CELSIUS
8
HOUR
To a solution of 1,4,6-trimethyl-1,4-dihydro-quinoxaline-2,3-dione (0.66 g, 3.2 mmol) in acetic acid (40 mL) was added bromine (0.52 g, 3.2 mmol) and the solution stirred at 50° C. overnight. The reaction mixture was cooled to room temperature and poured into water. The solution was neutralized with aqueous NaOH to Ph=...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2nccnc2c1
c1ccc2nccnc2c1
c1ccc2nccnc2c1
HBr
C(C)(=O)O
50
8
BrBr.Cc1ccc2c(c1)n(C)c(=O)c(=O)n2C>C(C)(=O)O>Cc1cc2c(cc1Br)n(C)c(=O)c(=O)n2C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-47389a4cedf14c17a95ffc3eefc86c4e
COc1cc2c(cc1C)C(C)(C)C(=O)N2Cc1ccccc1>>Cc1cc2c(cc1O)N(Cc1ccccc1)C(=O)C2(C)C
C(C1=CC=CC=C1)N1C(C(C2=CC(=C(C=C12)OC)C)(C)C)=O.B(Br)(Br)Br>>C(C1=CC=CC=C1)N1C(C(C2=CC(=C(C=C12)O)C)(C)C)=O
C[O:8][c:7]1[c:2]([CH3:1])[cH:3][c:4]2[c:5]([cH:6]1)[N:9]([CH2:10][c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1)[C:17](=[O:18])[C:19]2([CH3:20])[CH3:21]>>[CH3:1][c:2]1[cH:3][c:4]2[c:5]([cH:6][c:7]1[OH:8])[N:9]([CH2:10][c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1)[C:17](=[O:18])[C:19]2([CH3:20])[CH3:21]
COc1cc2c(cc1C)C(C)(C)C(=O)N2Cc1ccccc1
Cc1cc2c(cc1O)N(Cc1ccccc1)C(=O)C2(C)C
null
null
ClCCl
Deprotection
Cleavage of methoxy ethers to alcohols
c5320c7dfa4f544d4900efcae9b3262bf0d5286bcf39c86109232351f35b23d5
26a36596df80ec137b0e8087297418351c93c32819177f680675220622f215d4
O=C1Cc2ccccc2N1Cc1ccccc1
C-[O;H0;D2;+0:1]-[c:2](:[c:3]):[c:4]>>[OH;D1;+0:1]-[c:2](:[c:3]):[c:4]
93
[{"value": 93.0, "product": "C(C1=CC=CC=C1)N1C(C(C2=CC(=C(C=C12)O)C)(C)C)=O", "details": "PERCENTYIELD", "is_desired": false}]
-20
CELSIUS
8
HOUR
To a solution of 1-benzyl-6-methoxy-3,3,5-trimethyl-1,3-dihydro-indol-2-one (1.52 g, 5.15 mmol) in anhydrous dichloromethane (50 mL) was added slowly, under argon at −78° C., BBr3 (0.87 mL, 9.27 mmol). The reaction was warmed up to −20° C. and stirred overnight at room temperature. Water and the layer separated. The aq...
10.6084/m9.figshare.5104873.v1
null
Ether
Aromatic alcohol
null
null
c1ccccc1.c1ccc2c(c1)CC[NH]2
Other
ClCCl
-20
8
COc1cc2c(cc1C)C(C)(C)C(=O)N2Cc1ccccc1>ClCCl>Cc1cc2c(cc1O)N(Cc1ccccc1)C(=O)C2(C)C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-fbc489b022444d9881717fee9d6c961a
COc1cc(N(Cc2ccccc2)C(=O)C(C)C)c(Br)cc1C>>COc1cc2c(cc1C)C(C)(C)C(=O)N2Cc1ccccc1
[Cl-].[NH4+].C(C1=CC=CC=C1)N(C(C(C)C)=O)C1=C(C=C(C(=C1)OC)C)Br.CC(C)([O-])C.[Na+]>>C(C1=CC=CC=C1)N1C(C(C2=CC(=C(C=C12)OC)C)(C)C)=O
Br[c:6]1[c:5]([N:15]([C:13]([CH:10]([CH3:11])[CH3:12])=[O:14])[CH2:16][c:17]2[cH:18][cH:19][cH:20][cH:21][cH:22]2)[cH:4][c:3]([O:2][CH3:1])[c:8]([CH3:9])[cH:7]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([cH:7][c:8]1[CH3:9])[C:10]([CH3:11])([CH3:12])[C:13](=[O:14])[N:15]2[CH2:16][c:17]1[cH:18][cH:19][cH:20][cH:21][cH:22]1
COc1cc(N(Cc2ccccc2)C(=O)C(C)C)c(Br)cc1C
COc1cc2c(cc1C)C(C)(C)C(=O)N2Cc1ccccc1
null
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].C1(CCCCC1)P(C1CCCCC1)C1CCCCC1
O1CCOCC1
Functional Group Interconversion
OtherReaction
df1aa182059fb9257c102fb9f33a1d3c689b7330b48d169f061515a6fc482e69
56de34d4a44cb25d9380269ee5e138b0f24b40a3a0db22c5508049dc775a861f
O=C1Cc2ccccc2N1Cc1ccccc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[#7:5](-[C:6])-[C:7](=[O;D1;H0:8])-[CH;D3;+0:9](-[C;D1;H3:10])-[C;D1;H3:11]):[c:12]>>[C:6]-[#7:5]1-[C:7](=[O;D1;H0:8])-[C;H0;D4;+0:9](-[C;D1;H3:10])(-[C;D1;H3:11])-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]-1:[c:12]
57
[{"value": 57.0, "product": "C(C1=CC=CC=C1)N1C(C(C2=CC(=C(C=C12)OC)C)(C)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 56.8, "product": "C(C1=CC=CC=C1)N1C(C(C2=CC(=C(C=C12)OC)C)(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of N-benzyl-N-(2-bromo-5-methoxy-4-methyl-phenyl)-isobutyramide (4.35 g, 11.56 mmol) in 1,4-dioxane (115 mL) was added sodium tert-butoxide (1.66 g, 17.34 mmol). The mixture was degassed under argon for 30 minutes, then palladium (II) acetate (130 mg, 0.58 mmol) and tricyclohexylphosphine (162 mg, 0.58 mm...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1ccccc1
c1ccc2c(c1)CC[NH]2
c1ccc2c(c1)CC[NH]2.c1ccccc1
HBr
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].C1(CCCCC1)P(C1CCCCC1)C1CCCCC1.O1CCOCC1
null
null
COc1cc(N(Cc2ccccc2)C(=O)C(C)C)c(Br)cc1C>C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].C1(CCCCC1)P(C1CCCCC1)C1CCCCC1.O1CCOCC1>COc1cc2c(cc1C)C(C)(C)C(=O)N2Cc1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-702e68e33e77400490e5eec9993d467b
BrCc1ccccc1.COc1cc(NC(=O)C(C)C)c(Br)cc1C>>COc1cc(N(Cc2ccccc2)C(=O)C(C)C)c(Br)cc1C
O.BrC1=C(C=C(C(=C1)C)OC)NC(C(C)C)=O.[OH-].[K+].C(C1=CC=CC=C1)Br>>C(C1=CC=CC=C1)N(C(C(C)C)=O)C1=C(C=C(C(=C1)OC)C)Br
Br[CH2:7][c:8]1[cH:9][cH:10][cH:11][cH:12][cH:13]1.[CH3:1][O:2][c:3]1[cH:4][c:5]([NH:6][C:14](=[O:15])[CH:16]([CH3:17])[CH3:18])[c:19]([Br:20])[cH:21][c:22]1[CH3:23]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([N:6]([CH2:7][c:8]2[cH:9][cH:10][cH:11][cH:12][cH:13]2)[C:14](=[O:15])[CH:16]([CH3:17])[CH3:18])[c:19]([Br:20])[cH:21][c:22...
BrCc1ccccc1.COc1cc(NC(=O)C(C)C)c(Br)cc1C
COc1cc(N(Cc2ccccc2)C(=O)C(C)C)c(Br)cc1C
null
null
CS(=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
db9b1b8804b469c037e0a5ba95031d33e73dcd5fc2a6fa79163c623adf75f2a1
4a6c1e88c9e8bed487b746792f88d478ff36cc235f9a217d4632e6babdebdc9a
c1ccc(CNc2ccccc2)cc1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[C:5]-[C:6](=[O;D1;H0:7])-[NH;D2;+0:8]-[c:9](:[c:10]):[c:11]>>[C:5]-[C:6](=[O;D1;H0:7])-[N;H0;D3;+0:8](-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4])-[c:9](:[c:10]):[c:11]
99
[{"value": 99.0, "product": "C(C1=CC=CC=C1)N(C(C(C)C)=O)C1=C(C=C(C(=C1)OC)C)Br", "details": "PERCENTYIELD", "is_desired": false}, {"value": 98.9, "product": "C(C1=CC=CC=C1)N(C(C(C)C)=O)C1=C(C=C(C(=C1)OC)C)Br", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
5
MINUTE
A mixture of powdered KOH (1.3 g, 23.13 mmol) in DMSO (25 mL) was stirred at 0° C. for 5 minutes. N-(2-bromo-5-methoxy-4-methyl-phenyl)-isobutyramide (3.30 g, 11.56 mmol) was added cautiously followed immediately by the addition of benzylbromide (2.75 mL, 23.13 mmol) and the reaction stirred at room temperature for 48 ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amide
Tertiary amide
null
null
c1ccccc1.c1ccccc1
HBr
CS(=O)C
0
0.083333
BrCc1ccccc1.COc1cc(NC(=O)C(C)C)c(Br)cc1C>CS(=O)C>COc1cc(N(Cc2ccccc2)C(=O)C(C)C)c(Br)cc1C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-bce456ac6a614e5089098c99135f35ff
CC(C)C(=O)Cl.COc1cc(N)c(Br)cc1C>>COc1cc(NC(=O)C(C)C)c(Br)cc1C
BrC1=C(N)C=C(C(=C1)C)OC.[OH-].[K+].C(C(C)C)(=O)Cl>>BrC1=C(C=C(C(=C1)C)OC)NC(C(C)C)=O
Cl[C:7](=[O:8])[CH:9]([CH3:10])[CH3:11].[CH3:1][O:2][c:3]1[cH:4][c:5]([NH2:6])[c:12]([Br:13])[cH:14][c:15]1[CH3:16]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([NH:6][C:7](=[O:8])[CH:9]([CH3:10])[CH3:11])[c:12]([Br:13])[cH:14][c:15]1[CH3:16]
CC(C)C(=O)Cl.COc1cc(N)c(Br)cc1C
COc1cc(NC(=O)C(C)C)c(Br)cc1C
null
null
ClCCl
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
c1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])-[C;D1;H3:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[C;D1;H3:4]-[C:3](-[C;D1;H3:5])-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]
99.3
[{"value": 99.0, "product": "BrC1=C(C=C(C(=C1)C)OC)NC(C(C)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 99.3, "product": "BrC1=C(C=C(C(=C1)C)OC)NC(C(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
48
HOUR
To a biphasic mixture of 2-bromo-5-methoxy-4-methyl-aniline (5.6 g, 25.96 mmol), 10% KOH (27 mL) and dichloromethane (30 mL), was added dropwise isobutyryl chloride (3 mL, 28.55 mmol) in dichloromethane (10 mL). The reaction mixture was stirred at room temperature for 48 hrs. The layers were separated. The aqueous laye...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1ccccc1
HCl
ClCCl
null
48
CC(C)C(=O)Cl.COc1cc(N)c(Br)cc1C>ClCCl>COc1cc(NC(=O)C(C)C)c(Br)cc1C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-6ae525a6995242d69c3583ae30f02c03
COc1cc(N)ccc1C.[Br-]>>COc1cc(N)c(Br)cc1C
C(=O)(O)[O-].[Na+].COC=1C=C(N)C=CC1C.[Br-].[Br-].[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC.C(CCC)[N+](CCCC)(CCCC)CCCC.C(CCC)[N+](CCCC)(CCCC)CCCC>>BrC1=C(N)C=C(C(=C1)C)OC
[CH3:1][O:2][c:3]1[cH:4][c:5]([NH2:6])[cH:7][cH:9][c:10]1[CH3:11].[Br-:8]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([NH2:6])[c:7]([Br:8])[cH:9][c:10]1[CH3:11]
COc1cc(N)ccc1C.[Br-]
COc1cc(N)c(Br)cc1C
null
null
ClCCl
Functional Group Interconversion
Bromination
f6effe61353895b318215d8bd9b6bb1105cafbf7be8c217d748df587260b32c3
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1ccccc1
[Br-;H0;D0:1].[N;D1;H2:2]-[c:3](:[c:4]):[cH;D2;+0:5]:[c:6]:[c:7]>>[Br;H0;D1;+0:1]-[c;H0;D3;+0:5](:[c:6]:[c:7]):[c:3](-[N;D1;H2:2]):[c:4]
85.6
[{"value": 85.0, "product": "BrC1=C(N)C=C(C(=C1)C)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 85.6, "product": "BrC1=C(N)C=C(C(=C1)C)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2.5
HOUR
To a solution of 3-methoxy-4-methyl-aniline (8.19 g, 59.71 mmol) in dichloromethane (200 mL), was added tetrabutylammonium tribromide (28.79 g, 59.71 mmol) and the reaction mixture was stirred at room temperature for 2.5 hrs. Aqueous NaHCO3 was added and the layers separated. The aqueous layer was further extracted wit...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccccc1
c1ccccc1
c1ccccc1
null
ClCCl
null
2.5
COc1cc(N)ccc1C.[Br-]>ClCCl>COc1cc(N)c(Br)cc1C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c885315dcbe54d788919632571ee7f87
COc1cc([N+](=O)[O-])ccc1C>>COc1cc(N)ccc1C
CC1=C(C=C(C=C1)[N+](=O)[O-])OC.O.O.[Sn](Cl)Cl.C(=O)([O-])[O-].[K+].[K+]>>COC=1C=C(N)C=CC1C
O=[N+:6]([O-])[c:5]1[cH:4][c:3]([O:2][CH3:1])[c:9]([CH3:10])[cH:8][cH:7]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]([NH2:6])[cH:7][cH:8][c:9]1[CH3:10]
COc1cc([N+](=O)[O-])ccc1C
COc1cc(N)ccc1C
null
null
C(C)(=O)OCC.C(C)O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccccc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
86
[{"value": 86.0, "product": "COC=1C=C(N)C=CC1C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 84.5, "product": "COC=1C=C(N)C=CC1C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To a solution of 2-methyl-5-nitroanisole (11.56 g, 69.2 mmol) in a mixture of ethyl acetate (200 mL) and ethanol (70 mL) was added portionwise tin (II) chloride dihydrate (109 g, 0.483 mol) and the mixture was stirred at room temperature overnight. The reaction mixture was basified with aq. K2CO3 and filtered over celi...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1
Other
C(C)(=O)OCC.C(C)O
null
8
COc1cc([N+](=O)[O-])ccc1C>C(C)(=O)OCC.C(C)O>COc1cc(N)ccc1C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b5bf0860457b4e248df486a68c484723
CC(C)Cc1cc(Br)c2c(c1)C(C)(C)CO2.CC(C)OB(OC(C)C)OC(C)C>>CC(C)Cc1cc(B(O)O)c2c(c1)C(C)(C)CO2
Cl.[Li]CCCC.BrC1=CC(=CC=2C(COC21)(C)C)CC(C)C.C(C)(C)OB(OC(C)C)OC(C)C>>C(C(C)C)C=1C=C(C2=C(C(CO2)(C)C)C1)B(O)O
Br[c:7]1[cH:6][c:5]([CH2:4][CH:2]([CH3:1])[CH3:3])[cH:13][c:12]2[c:11]1[O:18][CH2:17][C:14]2([CH3:15])[CH3:16].CC(C)O[B:8]([O:9]C(C)C)[O:10]C(C)C>>[CH3:1][CH:2]([CH3:3])[CH2:4][c:5]1[cH:6][c:7]([B:8]([OH:9])[OH:10])[c:11]2[c:12]([cH:13]1)[C:14]([CH3:15])([CH3:16])[CH2:17][O:18]2
CC(C)Cc1cc(Br)c2c(c1)C(C)(C)CO2.CC(C)OB(OC(C)C)OC(C)C
CC(C)Cc1cc(B(O)O)c2c(c1)C(C)(C)CO2
null
null
C(C)(=O)OCC.C1CCOC1
Miscellaneous
Preparation of boronic acids
112c72bbe77af87a2ef270f9ef3e900f83a6ad272e2a1ee47eb37bf96c79880a
dafd25fbe01879c365f8c874026e570f49824f4bb82016b29d0c5d21aeb58ca3
c1ccc2c(c1)CCO2
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](:[c:5])-[#8:6]-[C:7].C-C(-C)-O-[B;H0;D3;+0:8](-[O;H0;D2;+0:9]-C(-C)-C)-[O;H0;D2;+0:10]-C(-C)-C>>[C:7]-[#8:6]-[c:4](:[c:5]):[c;H0;D3;+0:1](-[B;H0;D3;+0:8](-[OH;D1;+0:9])-[OH;D1;+0:10]):[c:2]:[c:3]
49.6
[{"value": 46.0, "product": "C(C(C)C)C=1C=C(C2=C(C(CO2)(C)C)C1)B(O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 49.6, "product": "C(C(C)C)C=1C=C(C2=C(C(CO2)(C)C)C1)B(O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-78
CELSIUS
5
MINUTE
To a mixture of 7-bromo-5-isobutyl-3,3-dimethyl-2,3-dihydro-benzofuran (9.9 g, 34.96 mmol) in THF (50 mL) cooled to −78° C. under an atmosphere of argon was added n-BuLi (25.17 mL, 2.5 M, 62.93 mmol) dropwise. The reaction mixture was stirred for 5 minutes and triisopropylborate (24.2 mL, 104.87 mmol) was added dropwis...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
Boronic acid
c1ccc2c(c1)CCO2
c1ccc2c(c1)CCO2
c1ccc2c(c1)CCO2
HBr
C(C)(=O)OCC.C1CCOC1
-78
0.083333
CC(C)Cc1cc(Br)c2c(c1)C(C)(C)CO2.CC(C)OB(OC(C)C)OC(C)C>C(C)(=O)OCC.C1CCOC1>CC(C)Cc1cc(B(O)O)c2c(c1)C(C)(C)CO2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-89cfa1cd693841edb6b03ec011fb8e03
CC(C)Cc1ccc2c(c1)C(C)(C)CO2.[Br-]>>CC(C)Cc1cc(Br)c2c(c1)C(C)(C)CO2
C(C(C)C)C=1C=CC2=C(C(CO2)(C)C)C1.[Br-].[Br-].[Br-].[NH+]1=CC=CC=C1.[NH+]1=CC=CC=C1.[NH+]1=CC=CC=C1>>BrC1=CC(=CC=2C(COC21)(C)C)CC(C)C
[CH3:1][CH:2]([CH3:3])[CH2:4][c:5]1[cH:6][cH:7][c:9]2[c:10]([cH:11]1)[C:12]([CH3:13])([CH3:14])[CH2:15][O:16]2.[Br-:8]>>[CH3:1][CH:2]([CH3:3])[CH2:4][c:5]1[cH:6][c:7]([Br:8])[c:9]2[c:10]([cH:11]1)[C:12]([CH3:13])([CH3:14])[CH2:15][O:16]2
CC(C)Cc1ccc2c(c1)C(C)(C)CO2.[Br-]
CC(C)Cc1cc(Br)c2c(c1)C(C)(C)CO2
null
null
ClCCl
Functional Group Interconversion
Bromination
8a5899f39c577ae2f5dbb7e89484f9814910050aa00e810b5c8bafb1acd06dbc
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1ccc2c(c1)CCO2
[Br-;H0;D0:1].[C:2]-[#8:3]-[c:4](:[c:5]):[cH;D2;+0:6]:[c:7]:[c:8]>>[Br;H0;D1;+0:1]-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:4](:[c:5])-[#8:3]-[C:2]
68.5
[{"value": 68.0, "product": "BrC1=CC(=CC=2C(COC21)(C)C)CC(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 68.5, "product": "BrC1=CC(=CC=2C(COC21)(C)C)CC(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To a solution of 5-isobutyl-3,3-dimethyl-2,3-dihydro-benzofuran (1.59 g, 7.78 mmol) in dichloromethane (40 mL) was added pyridinium tribromide (2.49 g, 7.78 mmol) and the reaction mixture stirred at room temperature overnight. The solution was washed with water and brine, dried (Mg2SO4), filtered and evaporated. The re...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2c(c1)CCO2
c1ccc2c(c1)CCO2
c1ccc2c(c1)CCO2
null
ClCCl
null
8
CC(C)Cc1ccc2c(c1)C(C)(C)CO2.[Br-]>ClCCl>CC(C)Cc1cc(Br)c2c(c1)C(C)(C)CO2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-901ce828923d41e8b5486673c213dff6
CC(C)C(O)c1ccc2c(c1)C(C)(C)CO2>>CC(C)Cc1ccc2c(c1)C(C)(C)CO2
O.FC(C(=O)O)(F)F.CC1(COC2=C1C=C(C=C2)C(C(C)C)O)C.C(C)[SiH](CC)CC>>C(C(C)C)C=1C=CC2=C(C(CO2)(C)C)C1
O[CH:4]([CH:2]([CH3:1])[CH3:3])[c:5]1[cH:6][cH:7][c:8]2[c:9]([cH:10]1)[C:11]([CH3:12])([CH3:13])[CH2:14][O:15]2>>[CH3:1][CH:2]([CH3:3])[CH2:4][c:5]1[cH:6][cH:7][c:8]2[c:9]([cH:10]1)[C:11]([CH3:12])([CH3:13])[CH2:14][O:15]2
CC(C)C(O)c1ccc2c(c1)C(C)(C)CO2
CC(C)Cc1ccc2c(c1)C(C)(C)CO2
null
null
ClCCl
Reduction
OtherReaction
3c5af32aa639db2ebe4d9851942e9468e1838e06ae5b2c1669bca1d5e0922c33
46f8a11b80b06e754a5a34198d843342612a5e7ede950bda52ce3a500cedba0b
c1ccc2c(c1)CCO2
O-[CH;D3;+0:1](-[C:2](-[C;D1;H3:3])-[C;D1;H3:4])-[c:5](:[c:6]):[c:7]>>[C;D1;H3:3]-[C:2](-[C;D1;H3:4])-[CH2;D2;+0:1]-[c:5](:[c:6]):[c:7]
87.7
[{"value": 87.0, "product": "C(C(C)C)C=1C=CC2=C(C(CO2)(C)C)C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 87.7, "product": "C(C(C)C)C=1C=CC2=C(C(CO2)(C)C)C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
10
MINUTE
To a cold solution (0° C.) of 1-(3,3-dimethyl-2,3-dihydro-benzofuran-5-yl)-2-methyl-propan-1-ol (1.97 g, 8.93 mmol) in dry dichloromethane (40 mL) was added triethylsilane (2.85 mL, 17.86 mmol). After 10 minutes, trifluoroacetic acid was the reaction mixture stirred at 0° C. for 30 minutes. Water was poured into the re...
10.6084/m9.figshare.5104873.v1
null
Secondary alcohol
null
null
null
c1ccc2c(c1)CCO2
Other
ClCCl
0
0.166667
CC(C)C(O)c1ccc2c(c1)C(C)(C)CO2>ClCCl>CC(C)Cc1ccc2c(c1)C(C)(C)CO2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-8ced0d5f185d429ab03b60c0c8ee990d
CC(C)C=O.CC1(C)COc2ccc(Br)cc21>>CC(C)C(O)c1ccc2c(c1)C(C)(C)CO2
[Cl-].[NH4+].C(C(C)C)=O.BrC=1C=CC2=C(C(CO2)(C)C)C1.[Li]CCCC>>CC1(COC2=C1C=C(C=C2)C(C(C)C)O)C
[CH3:1][CH:2]([CH3:3])[CH:4]=[O:5].Br[c:6]1[cH:7][cH:8][c:9]2[c:10]([cH:11]1)[C:12]([CH3:13])([CH3:14])[CH2:15][O:16]2>>[CH3:1][CH:2]([CH3:3])[CH:4]([OH:5])[c:6]1[cH:7][cH:8][c:9]2[c:10]([cH:11]1)[C:12]([CH3:13])([CH3:14])[CH2:15][O:16]2
CC(C)C=O.CC1(C)COc2ccc(Br)cc21
CC(C)C(O)c1ccc2c(c1)C(C)(C)CO2
null
null
C1CCOC1
C-C Coupling
Grignard_alcohol
a56606a78163c88dc4bf48a7c5ab26b38cb3fda591dd4b56afdf051b12beb5dd
1c0bd0afc1d5e370e3c8193faf738f03752295e40fa0eb99c756011e9a4be26b
c1ccc2c(c1)CCO2
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[C;D1;H3:6]-[C:7](-[C;D1;H3:8])-[CH;D2;+0:9]=[O;H0;D1;+0:10]>>[C;D1;H3:6]-[C:7](-[C;D1;H3:8])-[CH;D3;+0:9](-[OH;D1;+0:10])-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
106.7
[{"value": 100.0, "product": "CC1(COC2=C1C=C(C=C2)C(C(C)C)O)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 106.7, "product": "CC1(COC2=C1C=C(C=C2)C(C(C)C)O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
5
MINUTE
To a solution of 5-bromo-3,3-dimethyl-2,3-dihydro-benzofuran (2.03 g, 8.93 mmol) in dry THF (10 mL) at −78° C., under argon, was added dropwise n-BuLi (1.6 M in hexane, 13.4 mmol, 8.38 mL). The mixture was stirred for 5 minutes then isobutyraldehyde (1.22 mL, 8.38 mmol) was added and the mixture was slowly warmed up to...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aldehyde
Secondary alcohol
c1ccc2c(c1)CCO2
c1ccc2c(c1)CCO2
c1ccc2c(c1)CCO2
Br-
C1CCOC1
null
0.083333
CC(C)C=O.CC1(C)COc2ccc(Br)cc21>C1CCOC1>CC(C)C(O)c1ccc2c(c1)C(C)(C)CO2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-7a5800cb92e94a7ab363a3619bc4b26c
COc1ccc(Br)cc1C(C)(C)CCl>>CC1(C)COc2ccc(Br)cc21
BrC1=CC(=C(C=C1)OC)C(CCl)(C)C.Cl.N1=CC=CC=C1.N1=CC=CC2=CC=CC=C12>>BrC=1C=CC2=C(C(CO2)(C)C)C1
C[O:5][c:6]1[cH:7][cH:8][c:9]([Br:10])[cH:11][c:12]1[C:2]([CH3:1])([CH3:3])[CH2:4]Cl>>[CH3:1][C:2]1([CH3:3])[CH2:4][O:5][c:6]2[cH:7][cH:8][c:9]([Br:10])[cH:11][c:12]21
COc1ccc(Br)cc1C(C)(C)CCl
CC1(C)COc2ccc(Br)cc21
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
17eeb4763d9302b5045a1417df199ffda8f8cc9d73817017e66cab6c94957c5a
969a4609e178674696657c590a647839ca01abd1f90b8f0c9e475b1d6507651b
c1ccc2c(c1)CCO2
C-[O;H0;D2;+0:1]-[c:2](:[c:3]):[c:4]-[C:5](-[C;D1;H3:6])(-[C;D1;H3:7])-[CH2;D2;+0:8]-Cl>>[C;D1;H3:6]-[C:5]1(-[C;D1;H3:7])-[CH2;D2;+0:8]-[O;H0;D2;+0:1]-[c:2](:[c:3]):[c:4]-1
98
[{"value": 98.0, "product": "BrC=1C=CC2=C(C(CO2)(C)C)C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 97.9, "product": "BrC=1C=CC2=C(C(CO2)(C)C)C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 4-bromo-2-(2-chloro-1,1-dimethyl-ethyl)-1-methoxy-benzene (65 g, 0.234 mol), pyridine hydrochloride (121.8 g, 1.054 mol) and quinoline (110.67 mL, 0.936 mol) was refluxed at 164° C.–167° C. under argon for 5 hrs. After cooling to room temperature the reaction mixture was treated with ice-cold 6N HCl and ex...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ether
Ether
null
c1ccc2c(c1)CCO2
c1ccc2c(c1)CCO2
HCl
null
null
null
COc1ccc(Br)cc1C(C)(C)CCl>>CC1(C)COc2ccc(Br)cc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-6143f107a610417eb57f1701b3304807
C=C(C)CCl.COc1ccc(Br)cc1>>COc1ccc(Br)cc1C(C)(C)CCl
S(O)(O)(=O)=O.BrC1=CC=C(C=C1)OC.O.ClCC(=C)C>>BrC1=CC(=C(C=C1)OC)C(CCl)(C)C
[C:10]([CH3:11])(=[CH2:12])[CH2:13][Cl:14].[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([Br:7])[cH:8][cH:9]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([Br:7])[cH:8][c:9]1[C:10]([CH3:11])([CH3:12])[CH2:13][Cl:14]
C=C(C)CCl.COc1ccc(Br)cc1
COc1ccc(Br)cc1C(C)(C)CCl
null
null
ClCCl
C-C Coupling
Friedel-Crafts alkylation
f6021e53f57d07d48a856391b21137517c9bd669381174a55381b6219a6afd68
48297e5b607b4624d5b08506879ba8f9dd47fb272c10888542fa01ef83829ef2
c1ccccc1
[#8:1]-[c:2](:[c:3]):[cH;D2;+0:4]:[c:5]:[c:6].[C;D1;H3:7]-[C;H0;D3;+0:8](=[CH2;D1;+0:9])-[C:10]-[Cl;D1;H0:11]>>[#8:1]-[c:2](:[c:3]):[c;H0;D3;+0:4](-[C;H0;D4;+0:8](-[C;D1;H3:7])(-[CH3;D1;+0:9])-[C:10]-[Cl;D1;H0:11]):[c:5]:[c:6]
null
[]
null
null
null
null
Sulfuric acid (2 mL, 0.033 mol) was added dropwise under argon to 4-bromoanisole (14.6 mL, 0.117 mol). The mixture was warmed to 40–43° C. (warm water bath) and 3-chloro-2-methyl propene was added dropwise in 4 equal portions over 2 hrs. After 2 hrs at 40–43° C. the solution was diluted with dichloromethane and washed ...
10.6084/m9.figshare.5104873.v1
null
Vinyl
null
c1ccccc1
c1ccccc1
c1ccccc1
null
ClCCl
null
null
C=C(C)CCl.COc1ccc(Br)cc1>ClCCl>COc1ccc(Br)cc1C(C)(C)CCl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b9e5ce56ff19449393d82f4c2ca17317
CN(C)C(=O)c1cc(Br)c2c(c1)C(C)(C)CO2.O=Cc1ccc(OC(F)(F)F)c(Br)c1>>CN(C)C(=O)c1cc(-c2cc(C=O)ccc2OC(F)(F)F)c2c(c1)C(C)(C)CO2
C1(CCCCC1)P(C1=C(C=CC=C1)C1=CC=CC=C1)C1CCCCC1.[B]1OC(C(O1)(C)C)(C)C.BrC=1C=C(C=O)C=CC1OC(F)(F)F.C(C)N(CC)CC.CN(C(=O)C=1C=C(C2=C(C(CO2)(C)C)C1)Br)C>>CN(C(=O)C=1C=C(C2=C(C(CO2)(C)C)C1)C1=C(C=CC(=C1)C=O)OC(F)(F)F)C
Br[c:8]1[cH:7][c:6]([C:4]([N:2]([CH3:1])[CH3:3])=[O:5])[cH:24][c:23]2[c:22]1[O:29][CH2:28][C:25]2([CH3:26])[CH3:27].Br[c:9]1[cH:10][c:11]([CH:12]=[O:13])[cH:14][cH:15][c:16]1[O:17][C:18]([F:19])([F:20])[F:21]>>[CH3:1][N:2]([CH3:3])[C:4](=[O:5])[c:6]1[cH:7][c:8](-[c:9]2[cH:10][c:11]([CH:12]=[O:13])[cH:14][cH:15][c:16]2[...
CN(C)C(=O)c1cc(Br)c2c(c1)C(C)(C)CO2.O=Cc1ccc(OC(F)(F)F)c(Br)c1
CN(C)C(=O)c1cc(-c2cc(C=O)ccc2OC(F)(F)F)c2c(c1)C(C)(C)CO2
null
CC(=O)[O-].CC(=O)[O-].[Pd+2]
O1CCOCC1.O.C(C)(=O)OCC
C-C Coupling
Negishi
cb7e770ee1be461bb20a647f5f502c8c42a3886a14e9e2a7bc53a51bdf846d0a
a7a4ce9a92e2f8a62d28956a69a5cc384426ab72416e87d68c6a3feb23c22d66
c1ccc(-c2cccc3c2OCC3)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]-[C:4](-[#7:5])=[O;D1;H0:6]):[c:7](:[c:8])-[#8:9]-[C:10].Br-[c;H0;D3;+0:11](:[c:12]:[c:13]-[C:14]=[O;D1;H0:15]):[c:16](-[#8:17]):[c:18]>>[#7:5]-[C:4](=[O;D1;H0:6])-[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:11](:[c:12]:[c:13]-[C:14]=[O;D1;H0:15]):[c:16](-[#8:17]):[c:18]):[c:7](:[c:8])-[#8:9]-...
50
[{"value": 50.0, "product": "CN(C(=O)C=1C=C(C2=C(C(CO2)(C)C)C1)C1=C(C=CC(=C1)C=O)OC(F)(F)F)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 44.4, "product": "CN(C(=O)C=1C=C(C2=C(C(CO2)(C)C)C1)C1=C(C=CC(=C1)C=O)OC(F)(F)F)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
null
null
To a solution of 7-bromo-3,3-dimethyl-2,3-dihydro-benzofuran-5-carboxylic acid dimethylamide (437 mg, 1.46 mmol) in dioxane (4 mL), were added under argon, triethylamine (0.82 mL, 5.86 mmol), Pd(OAc)2 (16 mg, 0.07 mmol), 2-(dicyclohexylphosphino)biphenyl (103 mg, 0.29 mmol) and pinacolborane (0.64 mL, 4.40 mmol) dropwi...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide
null
c1ccc2c(c1)CCO2.c1ccccc1
c1ccccc1.c1ccc2c(c1)CCO2
c1ccccc1.c1ccc2c(c1)CCO2
Br-
CC(=O)[O-].CC(=O)[O-].[Pd+2].O1CCOCC1.O.C(C)(=O)OCC
80
null
CN(C)C(=O)c1cc(Br)c2c(c1)C(C)(C)CO2.O=Cc1ccc(OC(F)(F)F)c(Br)c1>CC(=O)[O-].CC(=O)[O-].[Pd+2].O1CCOCC1.O.C(C)(=O)OCC>CN(C)C(=O)c1cc(-c2cc(C=O)ccc2OC(F)(F)F)c2c(c1)C(C)(C)CO2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-cc5fd901768f4887b9c9ef8595d7ca2c
CC(C)(C)OC(=O)Nc1ccccc1N.COC(=O)c1ccc(C(=O)O)s1>>COC(=O)c1ccc(C(=O)Nc2ccccc2NC(=O)OC(C)(C)C)s1
C(=O)(N1C=NC=C1)N1C=NC=C1.COC(=O)C=1SC(=CC1)C(=O)O.C(C)(C)(C)OC(NC1=C(C=CC=C1)N)=O>>COC(=O)C=1SC(=CC1)C(NC1=C(C=CC=C1)NC(=O)OC(C)(C)C)=O
[NH2:11][c:12]1[cH:13][cH:14][cH:15][cH:16][c:17]1[NH:18][C:19](=[O:20])[O:21][C:22]([CH3:23])([CH3:24])[CH3:25].O[C:9]([c:8]1[cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[s:26]1)=[O:10]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([C:9](=[O:10])[NH:11][c:12]2[cH:13][cH:14][cH:15][cH:16][c:17]2[NH:18][C:19](=[O:20]...
CC(C)(C)OC(=O)Nc1ccccc1N.COC(=O)c1ccc(C(=O)O)s1
COC(=O)c1ccc(C(=O)Nc2ccccc2NC(=O)OC(C)(C)C)s1
null
null
C1CCOC1
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1ccccc1)c1cccs1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#16;a:5]:[c:6]-[C:7](-[#8:8])=[O;D1;H0:9].[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[#8:8]-[C:7](=[O;D1;H0:9])-[c:6]:[#16;a:5]:[c:3](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13]):[c:4]
80.2
[{"value": 80.2, "product": "COC(=O)C=1SC(=CC1)C(NC1=C(C=CC=C1)NC(=O)OC(C)(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
Under an argon atmosphere 21.0 g (129 mmol) carbonyldiimidazol was added to a solution of 24.1 g (129 mmol) thiophene-2,5-dicarboxylic acid monomethyl ester in 600 ml THF. After 2 h at rt 26.9 g (129 mmol) (2-amino-phenyl)-carbamic acid tert-butyl ester were added and the reaction mixture was stirred for further 4 h at...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccsc1.c1ccccc1
HO-
C1CCOC1
null
4
CC(C)(C)OC(=O)Nc1ccccc1N.COC(=O)c1ccc(C(=O)O)s1>C1CCOC1>COC(=O)c1ccc(C(=O)Nc2ccccc2NC(=O)OC(C)(C)C)s1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-fe083d7fc1964a5597f6c4073c73ab34
COC(=O)c1ccc(C(=O)Nc2ccccc2NC(=O)OC(C)(C)C)s1>>CC(C)(C)OC(=O)Nc1ccccc1NC(=O)c1ccc(C(=O)O)s1
COC(=O)C=1SC(=CC1)C(NC1=C(C=CC=C1)NC(=O)OC(C)(C)C)=O.[OH-].[K+]>>C(C)(C)(C)OC(=O)NC1=C(C=CC=C1)NC(=O)C1=CC=C(S1)C(=O)O
C[O:24][C:22]([c:21]1[cH:20][cH:19][c:18]([C:16]([NH:15][c:14]2[c:9]([NH:8][C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[cH:10][cH:11][cH:12][cH:13]2)=[O:17])[s:25]1)=[O:23]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[NH:8][c:9]1[cH:10][cH:11][cH:12][cH:13][c:14]1[NH:15][C:16](=[O:17])[c:18]1[cH:19][cH:20][c:...
COC(=O)c1ccc(C(=O)Nc2ccccc2NC(=O)OC(C)(C)C)s1
CC(C)(C)OC(=O)Nc1ccccc1NC(=O)c1ccc(C(=O)O)s1
null
null
O.CO
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=C(Nc1ccccc1)c1cccs1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#16;a:5]>>[#16;a:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
80
[{"value": 80.0, "product": "C(C)(C)(C)OC(=O)NC1=C(C=CC=C1)NC(=O)C1=CC=C(S1)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
DAY
To a suspension of 18.5 g (50 mmol) 5-(2-tert-Butoxycarbonylamino-phenyl-carbamoyl)-thiophene-2-carboxylic acid methyl ester in 500 ml MeOH was added within 20 minutes a solution of 5.6 g (100 mmol) potassium hydroxide in 100 ml water. The reaction mixture was stirred at room temperature for 2 d. The MeOH was evaporate...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccsc1
Other
O.CO
null
48
COC(=O)c1ccc(C(=O)Nc2ccccc2NC(=O)OC(C)(C)C)s1>O.CO>CC(C)(C)OC(=O)Nc1ccccc1NC(=O)c1ccc(C(=O)O)s1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a2cea9a32b0044a881f3c9217467f865
CC(C)(C)OC(=O)Nc1ccccc1NC(=O)c1ccc(C(=O)O)s1.CCCC(C)N>>CCCC(C)NC(=O)c1ccc(C(=O)Nc2ccccc2NC(=O)OC(C)(C)C)s1
CC(CCC)N.C(C)(C)(C)OC(=O)NC1=C(C=CC=C1)NC(=O)C1=CC=C(S1)C(=O)O.C(=O)(N1C=NC=C1)N1C=NC=C1>>C(C)(C)(C)OC(NC1=C(C=CC=C1)NC(=O)C=1SC(=CC1)C(NC(CCC)C)=O)=O
O[C:7](=[O:8])[c:9]1[cH:10][cH:11][c:12]([C:13](=[O:14])[NH:15][c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[NH:22][C:23](=[O:24])[O:25][C:26]([CH3:27])([CH3:28])[CH3:29])[s:30]1.[CH3:1][CH2:2][CH2:3][CH:4]([CH3:5])[NH2:6]>>[CH3:1][CH2:2][CH2:3][CH:4]([CH3:5])[NH:6][C:7](=[O:8])[c:9]1[cH:10][cH:11][c:12]([C:13](=[O:14])[N...
CC(C)(C)OC(=O)Nc1ccccc1NC(=O)c1ccc(C(=O)O)s1.CCCC(C)N
CCCC(C)NC(=O)c1ccc(C(=O)Nc2ccccc2NC(=O)OC(C)(C)C)s1
null
null
C1CCOC1
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Nc1ccccc1)c1cccs1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#16;a:5]:[c:6]-[C:7](-[#7:8])=[O;D1;H0:9].[C:10]-[C:11](-[C;D1;H3:12])-[NH2;D1;+0:13]>>[#7:8]-[C:7](=[O;D1;H0:9])-[c:6]:[#16;a:5]:[c:3](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:13]-[C:11](-[C:10])-[C;D1;H3:12]):[c:4]
null
[]
45
CELSIUS
1
HOUR
To a solution of 4.4 g (12.1 mmol) 5-(2-tert-butoxycarbonylamino-phenylcarbamoyl)-thiophene-2-carboxylic acid in 80 ml THF were added 2.2 g (13.6 mmol) carbonyldiimidazol. The reaction mixture was stirred at 45° C. for 1 h and then cooled to rt. After addition of 1.05 g (12 mmol) 2-pentylamine the reaction mixture was ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccsc1.c1ccccc1
HO-
C1CCOC1
45
1
CC(C)(C)OC(=O)Nc1ccccc1NC(=O)c1ccc(C(=O)O)s1.CCCC(C)N>C1CCOC1>CCCC(C)NC(=O)c1ccc(C(=O)Nc2ccccc2NC(=O)OC(C)(C)C)s1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d54340666b7148d9a6bdec48400dbcf4
CC(C)N(CCN)C(C)C.COC(=O)c1ccc(C(=O)[O-])nc1>>COC(=O)c1ccc(C(=O)NCCN(C(C)C)C(C)C)nc1
COC(=O)C=1C=CC(=NC1)C(=O)[O-].[K+].S(=O)(Cl)Cl.C(C)(C)N(CCN)C(C)C.C(C)N(CC)CC>>COC(C1=CN=C(C=C1)C(NCCN(C(C)C)C(C)C)=O)=O
[NH2:11][CH2:12][CH2:13][N:14]([CH:15]([CH3:16])[CH3:17])[CH:18]([CH3:19])[CH3:20].[O-][C:9]([c:8]1[cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:22][n:21]1)=[O:10]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([C:9](=[O:10])[NH:11][CH2:12][CH2:13][N:14]([CH:15]([CH3:16])[CH3:17])[CH:18]([CH3:19])[CH3:20])[n:21][c...
CC(C)N(CCN)C(C)C.COC(=O)c1ccc(C(=O)[O-])nc1
COC(=O)c1ccc(C(=O)NCCN(C(C)C)C(C)C)nc1
null
null
ClC(C)Cl.C(Cl)Cl.CN(C)C=O
Acylation
OtherReaction
01b411aa709aa72475efefee2037796aeb41c60940ddba8e15aefc45a95317a8
45ca336cc0b18cf59a837ab710e8845f67d23306b24bf1f37b36a34a2de4779a
c1ccncc1
[C:1]-[C:2]-[NH2;D1;+0:3].[O-]-[C;H0;D3;+0:4](=[O;D1;H0:5])-[c:6](:[c:7]):[#7;a:8]:[c:9]>>[C:1]-[C:2]-[NH;D2;+0:3]-[C;H0;D3;+0:4](=[O;D1;H0:5])-[c:6](:[c:7]):[#7;a:8]:[c:9]
74
[{"value": 74.0, "product": "COC(C1=CN=C(C=C1)C(NCCN(C(C)C)C(C)C)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
12
HOUR
A suspension of 1.1 g (5 mmol) potassium 5-methoxycarbonyl-pyridine-2-carboxylate, 0.9 ml (12 mmol) thionyl chloride and 0.1 ml DMF in 5 ml dichloroethane was heated at reflux for 2 h. To the reaction mixture 5 ml CH2Cl2 were added and the solvent was evaporated. This procedure was repeated three times. The residue was...
10.6084/m9.figshare.5104873.v1
null
Primary amine
Secondary amide
null
null
c1ccncc1
HO-
ClC(C)Cl.C(Cl)Cl.CN(C)C=O
null
12
CC(C)N(CCN)C(C)C.COC(=O)c1ccc(C(=O)[O-])nc1>ClC(C)Cl.C(Cl)Cl.CN(C)C=O>COC(=O)c1ccc(C(=O)NCCN(C(C)C)C(C)C)nc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-32090cdb0df14200be7298a12d733dd7
COC(=O)c1ccc(C(=O)NCCN(C(C)C)C(C)C)nc1>>CC(C)N(CCNC(=O)c1ccc(C(=O)O)cn1)C(C)C
COC(C1=CN=C(C=C1)C(NCCN(C(C)C)C(C)C)=O)=O.[OH-].[Na+]>>C(C)(C)N(CCNC(=O)C1=NC=C(C(=O)O)C=C1)C(C)C
C[O:16][C:14]([c:13]1[cH:12][cH:11][c:10]([C:8]([NH:7][CH2:6][CH2:5][N:4]([CH:2]([CH3:1])[CH3:3])[CH:19]([CH3:20])[CH3:21])=[O:9])[n:18][cH:17]1)=[O:15]>>[CH3:1][CH:2]([CH3:3])[N:4]([CH2:5][CH2:6][NH:7][C:8](=[O:9])[c:10]1[cH:11][cH:12][c:13]([C:14](=[O:15])[OH:16])[cH:17][n:18]1)[CH:19]([CH3:20])[CH3:21]
COC(=O)c1ccc(C(=O)NCCN(C(C)C)C(C)C)nc1
CC(C)N(CCNC(=O)c1ccc(C(=O)O)cn1)C(C)C
null
null
CO.C1CCOC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccncc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]:[#7;a:6]>>[#7;a:6]:[c:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
88.9
[{"value": 88.9, "product": "C(C)(C)N(CCNC(=O)C1=NC=C(C(=O)O)C=C1)C(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of 1100 mg (3.6 mmol) 6-(2-diisopropylamino-ethylcarbamoyl)-nicotinic acid methyl ester in 10 ml THF and 3.0 ml MeOH was added 3.6 ml of an 2N aqueous NaOH solution. After 4 h at rt the solvent was evaporated. The residue was acidified with 1N HCl, filtered off and washed with water to give 936 mg (3.2 mm...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccncc1
Other
CO.C1CCOC1
null
null
COC(=O)c1ccc(C(=O)NCCN(C(C)C)C(C)C)nc1>CO.C1CCOC1>CC(C)N(CCNC(=O)c1ccc(C(=O)O)cn1)C(C)C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c68c8c1c71e8490ca4bfbc32fb5643b0
COC(=O)c1ccc(N)c(S(C)(=O)=O)c1.Cc1c(S(=O)(=O)Cl)sc2ccc(Cl)cc12>>COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(Cl)cc3c2C)c(S(C)(=O)=O)c1
ClC1=CC2=C(SC(=C2C)S(=O)(=O)Cl)C=C1.C1CCOC1.NC1=C(C=C(C(=O)OC)C=C1)S(=O)(=O)C.[H-].[Na+].[H-].[Na+]>>ClC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C(=O)OC)C=C2)S(=O)(=O)C)C=C1
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([NH2:9])[c:24]([S:25]([CH3:26])(=[O:27])=[O:28])[cH:29]1.Cl[S:10](=[O:11])(=[O:12])[c:13]1[s:14][c:15]2[cH:16][cH:17][c:18]([Cl:19])[cH:20][c:21]2[c:22]1[CH3:23]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([NH:9][S:10](=[O:11])(=[O:12])[c:13]2[s:14][c:15]3[cH:16][c...
COC(=O)c1ccc(N)c(S(C)(=O)=O)c1.Cc1c(S(=O)(=O)Cl)sc2ccc(Cl)cc12
COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(Cl)cc3c2C)c(S(C)(=O)=O)c1
null
null
CN(C)C=O
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=S(=O)(Nc1ccccc1)c1cc2ccccc2s1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[#16;a:6]:[c:7].[NH2;D1;+0:8]-[c:9](:[c:10]):[c:11]>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[NH;D2;+0:8]-[c:9](:[c:10]):[c:11])-[c:4](:[c:5]):[#16;a:6]:[c:7]
44.7
[{"value": 44.7, "product": "ClC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C(=O)OC)C=C2)S(=O)(=O)C)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
Into a mixed solvent of 20 mL of THF and 3 mL of DMF was dissolved 985 mg of methyl 4-amino-3-methanesulfonylbenzoate, followed by addition of 170 mg of sodium hydride (oily, 60%) at 0° C. After 20 minutes of stirring at the same temperature, 1.28 g of 5-chloro-2-chlorosulfonyl-3-methylbenzo[b]thiophene was added at 0°...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccccc1.c1ccc2sccc2c1
HCl
CN(C)C=O
null
1
COC(=O)c1ccc(N)c(S(C)(=O)=O)c1.Cc1c(S(=O)(=O)Cl)sc2ccc(Cl)cc12>CN(C)C=O>COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(Cl)cc3c2C)c(S(C)(=O)=O)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a152e2c19d984a5485caa2e2058b994e
COC(=O)c1cc(S(C)(=O)=O)c(N)cc1C.Cc1c(S(=O)(=O)Cl)sc2ccc(Cl)cc12>>COC(=O)c1cc(S(C)(=O)=O)c(NS(=O)(=O)c2sc3ccc(Cl)cc3c2C)cc1C
ClC1=CC2=C(SC(=C2C)S(=O)(=O)Cl)C=C1.[H-].[Na+].ClC1=CC2=C(SC(=C2C)S(=O)(=O)Cl)C=C1.C1CCOC1.NC1=CC(=C(C(=O)OC)C=C1S(=O)(=O)C)C.[H-].[Na+]>>ClC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=CC(=C(C(=O)OC)C=C2S(=O)(=O)C)C)C=C1
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([S:8]([CH3:9])(=[O:10])=[O:11])[c:12]([NH2:13])[cH:28][c:29]1[CH3:30].Cl[S:14](=[O:15])(=[O:16])[c:17]1[s:18][c:19]2[cH:20][cH:21][c:22]([Cl:23])[cH:24][c:25]2[c:26]1[CH3:27]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([S:8]([CH3:9])(=[O:10])=[O:11])[c:12]([NH:13][S:14](=[O:15...
COC(=O)c1cc(S(C)(=O)=O)c(N)cc1C.Cc1c(S(=O)(=O)Cl)sc2ccc(Cl)cc12
COC(=O)c1cc(S(C)(=O)=O)c(NS(=O)(=O)c2sc3ccc(Cl)cc3c2C)cc1C
null
null
CN(C)C=O
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=S(=O)(Nc1ccccc1)c1cc2ccccc2s1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[#16;a:6]:[c:7].[NH2;D1;+0:8]-[c:9](:[c:10]):[c:11]>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[NH;D2;+0:8]-[c:9](:[c:10]):[c:11])-[c:4](:[c:5]):[#16;a:6]:[c:7]
45.2
[{"value": 45.2, "product": "ClC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=CC(=C(C(=O)OC)C=C2S(=O)(=O)C)C)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
Into 10 mL of THF was dissolved 135 mg of methyl 4-amino-5-methanesulfonyl-2-methylbenzoate, followed by addition of 22 mg of sodium hydride (oily, 60%) at room temperature. After 20 minutes of stirring at the same temperature, 130 mg of 5-chloro-2-chlorosulfonyl-3-methylbenzo[b]thiophene was added at 0° C., followed b...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccccc1.c1ccc2sccc2c1
HCl
CN(C)C=O
null
1
COC(=O)c1cc(S(C)(=O)=O)c(N)cc1C.Cc1c(S(=O)(=O)Cl)sc2ccc(Cl)cc12>CN(C)C=O>COC(=O)c1cc(S(C)(=O)=O)c(NS(=O)(=O)c2sc3ccc(Cl)cc3c2C)cc1C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-46eef5de2b1e4935b5dd697656646385
COC(=O)c1ccc(N)c(C(=O)OC)c1.Cc1c(S(=O)(=O)Cl)sc2ccc(Cl)cc12>>COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(Cl)cc3c2C)c(C(=O)OC)c1
[H-].[Na+].NC1=C(C=C(C(=O)OC)C=C1)C(=O)OC.[H-].[Na+].ClC1=CC2=C(SC(=C2C)S(=O)(=O)Cl)C=C1>>ClC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C(=O)OC)C=C2)C(=O)OC)C=C1
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([NH2:9])[c:24]([C:25](=[O:26])[O:27][CH3:28])[cH:29]1.Cl[S:10](=[O:11])(=[O:12])[c:13]1[s:14][c:15]2[cH:16][cH:17][c:18]([Cl:19])[cH:20][c:21]2[c:22]1[CH3:23]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([NH:9][S:10](=[O:11])(=[O:12])[c:13]2[s:14][c:15]3[cH:16][cH:1...
COC(=O)c1ccc(N)c(C(=O)OC)c1.Cc1c(S(=O)(=O)Cl)sc2ccc(Cl)cc12
COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(Cl)cc3c2C)c(C(=O)OC)c1
null
null
C1CCOC1
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=S(=O)(Nc1ccccc1)c1cc2ccccc2s1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[#16;a:6]:[c:7].[#8:8]-[C:9](=[O;D1;H0:10])-[c:11]:[c:12](-[NH2;D1;+0:13]):[c:14]>>[#8:8]-[C:9](=[O;D1;H0:10])-[c:11]:[c:12](-[NH;D2;+0:13]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[#16;a:6]:[c:7]):[c:14]
29.5
[{"value": 29.5, "product": "ClC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C(=O)OC)C=C2)C(=O)OC)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
20
MINUTE
Into 8 mL of THF was dissolved 115 mg of dimethyl 4-aminoisophthalate, followed by addition of 22 mg of sodium hydride (oily, 60%). After 20 minutes of stirring at room temperature, 130 mg of 5-chloro-2-chlorosulfonyl-3-methylbenzo[b]thiophene was added at the same temperature, followed by 30 minutes of stirring at roo...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccccc1.c1ccc2sccc2c1
HCl
C1CCOC1
null
0.333333
COC(=O)c1ccc(N)c(C(=O)OC)c1.Cc1c(S(=O)(=O)Cl)sc2ccc(Cl)cc12>C1CCOC1>COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(Cl)cc3c2C)c(C(=O)OC)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-6ae174be5f614c5994a1b87d3f53b153
COC(=O)c1ccc(N)c(OC)c1.Cc1c(S(=O)(=O)Cl)sc2ccc(Cl)cc12>>COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(Cl)cc3c2C)c(OC)c1
NC1=C(C=C(C(=O)OC)C=C1)OC.ClC1=CC2=C(SC(=C2C)S(=O)(=O)Cl)C=C1>>ClC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C(=O)OC)C=C2)OC)C=C1
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([NH2:9])[c:24]([O:25][CH3:26])[cH:27]1.Cl[S:10](=[O:11])(=[O:12])[c:13]1[s:14][c:15]2[cH:16][cH:17][c:18]([Cl:19])[cH:20][c:21]2[c:22]1[CH3:23]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([NH:9][S:10](=[O:11])(=[O:12])[c:13]2[s:14][c:15]3[cH:16][cH:17][c:18]([Cl:19...
COC(=O)c1ccc(N)c(OC)c1.Cc1c(S(=O)(=O)Cl)sc2ccc(Cl)cc12
COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(Cl)cc3c2C)c(OC)c1
null
null
N1=CC=CC=C1
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=S(=O)(Nc1ccccc1)c1cc2ccccc2s1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[#16;a:6]:[c:7].[NH2;D1;+0:8]-[c:9](:[c:10]):[c:11]>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[NH;D2;+0:8]-[c:9](:[c:10]):[c:11])-[c:4](:[c:5]):[#16;a:6]:[c:7]
48.4
[{"value": 48.4, "product": "ClC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C(=O)OC)C=C2)OC)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
14
HOUR
Into 4 mL of pyridine were dissolved 120 mg of methyl 4-amino-3-methoxybenzoate and 150 mg of 5-chloro-2-chlorosulfonyl-3-methylbenzo[b]thiophene, followed by 14 hours of stirring at room temperature. After confirmation of disappearance of the starting material, the reaction was terminated by adding water at 0° C., fol...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccccc1.c1ccc2sccc2c1
HCl
N1=CC=CC=C1
null
14
COC(=O)c1ccc(N)c(OC)c1.Cc1c(S(=O)(=O)Cl)sc2ccc(Cl)cc12>N1=CC=CC=C1>COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(Cl)cc3c2C)c(OC)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d655178a714a49b1b6bcea7037858048
COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(Cl)cc3c2C)c(S(C)(=O)=O)c1>>Cc1c(S(=O)(=O)Nc2ccc(CO)cc2S(C)(=O)=O)sc2ccc(Cl)cc12
[H-].C(C(C)C)[Al+]CC(C)C.ClC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C(=O)OC)C=C2)S(=O)(=O)C)C=C1>>ClC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)CO)S(=O)(=O)C)C=C1
CO[C:12]([c:11]1[cH:10][cH:9][c:8]([NH:7][S:4]([c:3]2[c:2]([CH3:1])[c:27]3[c:21]([s:20]2)[cH:22][cH:23][c:24]([Cl:25])[cH:26]3)(=[O:5])=[O:6])[c:15]([S:16]([CH3:17])(=[O:18])=[O:19])[cH:14]1)=[O:13]>>[CH3:1][c:2]1[c:3]([S:4](=[O:5])(=[O:6])[NH:7][c:8]2[cH:9][cH:10][c:11]([CH2:12][OH:13])[cH:14][c:15]2[S:16]([CH3:17])(=...
COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(Cl)cc3c2C)c(S(C)(=O)=O)c1
Cc1c(S(=O)(=O)Nc2ccc(CO)cc2S(C)(=O)=O)sc2ccc(Cl)cc12
null
null
C1(=CC=CC=C1)C
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
O=S(=O)(Nc1ccccc1)c1cc2ccccc2s1
C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3](:[c:4]):[c:5]>>[OH;D1;+0:2]-[CH2;D2;+0:1]-[c:3](:[c:4]):[c:5]
80.1
[{"value": 80.1, "product": "ClC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)CO)S(=O)(=O)C)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-78
CELSIUS
20
MINUTE
Into 10 mL of toluene was dissolved 305 mg of Compound 1, and the solution was cooled to −78° C., followed by addition of 2.2 mL of 1.01 mol/L toluene solution of diisobutylaluminum hydride. After 20 minutes of stirring at the same temperature, the mixture was gradually warmed to 0° C. and stirred for 1 hour. After the...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
c1ccccc1.c1ccc2sccc2c1
Other
C1(=CC=CC=C1)C
-78
0.333333
COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(Cl)cc3c2C)c(S(C)(=O)=O)c1>C1(=CC=CC=C1)C>Cc1c(S(=O)(=O)Nc2ccc(CO)cc2S(C)(=O)=O)sc2ccc(Cl)cc12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e7b088af0aa04e6893ff19a8160fc6c1
CCOC(=O)c1ccc(N)cc1.Cc1c(S(=O)(=O)Cl)sc2ccc(Cl)cc12>>CCOC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(Cl)cc3c2C)cc1
NC1=CC=C(C(=O)OCC)C=C1.ClC1=CC2=C(SC(=C2C)S(=O)(=O)Cl)C=C1.Cl>>ClC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=CC=C(C(=O)OCC)C=C2)C=C1
[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][c:9]([NH2:10])[cH:25][cH:26]1.Cl[S:11](=[O:12])(=[O:13])[c:14]1[s:15][c:16]2[cH:17][cH:18][c:19]([Cl:20])[cH:21][c:22]2[c:23]1[CH3:24]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][c:9]([NH:10][S:11](=[O:12])(=[O:13])[c:14]2[s:15][c:16]3[cH:17][cH:18][c:19]([Cl:2...
CCOC(=O)c1ccc(N)cc1.Cc1c(S(=O)(=O)Cl)sc2ccc(Cl)cc12
CCOC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(Cl)cc3c2C)cc1
null
null
N1=CC=CC=C1
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=S(=O)(Nc1ccccc1)c1cc2ccccc2s1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[#16;a:6]:[c:7].[NH2;D1;+0:8]-[c:9](:[c:10]):[c:11]>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[NH;D2;+0:8]-[c:9](:[c:10]):[c:11])-[c:4](:[c:5]):[#16;a:6]:[c:7]
53.7
[{"value": 53.7, "product": "ClC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=CC=C(C(=O)OCC)C=C2)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
Into 3 mL of pyridine was dissolved 60 mg of ethyl 4-aminobenzoate, and 123 mg of 5-chloro-2-chlorosulfonyl-3-methylbenzo[b]thiophene was added at 0° C., followed by 2 hours of stirring at room temperature. After confirmation of disappearance of the starting material, 2 mol/L hydrochloric acid was added, followed by ex...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccccc1.c1ccc2sccc2c1
HCl
N1=CC=CC=C1
null
2
CCOC(=O)c1ccc(N)cc1.Cc1c(S(=O)(=O)Cl)sc2ccc(Cl)cc12>N1=CC=CC=C1>CCOC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(Cl)cc3c2C)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-45831d6810984499afc47944b982521b
COC(=O)c1ccc(N)c(S(C)(=O)=O)c1.Cc1c(S(=O)(=O)Cl)sc2ccc(F)cc12>>COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(F)cc3c2C)c(S(C)(=O)=O)c1
[H-].[Na+].NC1=C(C=C(C(=O)OC)C=C1)S(=O)(=O)C.ClS(=O)(=O)C1=C(C2=C(S1)C=CC(=C2)F)C>>FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C(=O)OC)C=C2)S(=O)(=O)C)C=C1
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([NH2:9])[c:24]([S:25]([CH3:26])(=[O:27])=[O:28])[cH:29]1.Cl[S:10](=[O:11])(=[O:12])[c:13]1[s:14][c:15]2[cH:16][cH:17][c:18]([F:19])[cH:20][c:21]2[c:22]1[CH3:23]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([NH:9][S:10](=[O:11])(=[O:12])[c:13]2[s:14][c:15]3[cH:16][cH...
COC(=O)c1ccc(N)c(S(C)(=O)=O)c1.Cc1c(S(=O)(=O)Cl)sc2ccc(F)cc12
COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(F)cc3c2C)c(S(C)(=O)=O)c1
null
null
C1CCOC1
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=S(=O)(Nc1ccccc1)c1cc2ccccc2s1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[#16;a:6]:[c:7].[NH2;D1;+0:8]-[c:9](:[c:10]):[c:11]>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[NH;D2;+0:8]-[c:9](:[c:10]):[c:11])-[c:4](:[c:5]):[#16;a:6]:[c:7]
89.7
[{"value": 89.7, "product": "FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C(=O)OC)C=C2)S(=O)(=O)C)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
Into 300 mL of THF was dissolved 14.0 g of methyl 4-amino-3-methanesulfonylbenzoate, followed by addition of 6.10 g of sodium hydride (oily, 60%) at 0° C. After 40 minutes of stirring at the same temperature, 16.0 g of 2-chlorosulfonyl-5-fluoro-3-methylbenzo[b]thiophene was added at 0° C., followed by 3 hours of stirri...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccccc1.c1ccc2sccc2c1
HCl
C1CCOC1
null
3
COC(=O)c1ccc(N)c(S(C)(=O)=O)c1.Cc1c(S(=O)(=O)Cl)sc2ccc(F)cc12>C1CCOC1>COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(F)cc3c2C)c(S(C)(=O)=O)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b427e01b17ac4285894a0f804cc42901
COC(=O)c1ccc(N)c(S(C)(=O)=O)c1.Cc1ccc2sc(S(=O)(=O)Cl)c(C)c2c1>>COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(C)cc3c2C)c(S(C)(=O)=O)c1
[H-].[Na+].NC1=C(C=C(C(=O)OC)C=C1)S(=O)(=O)C.ClS(=O)(=O)C1=C(C2=C(S1)C=CC(=C2)C)C>>CC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C(=O)OC)C=C2)S(=O)(=O)C)C=C1
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([NH2:9])[c:24]([S:25]([CH3:26])(=[O:27])=[O:28])[cH:29]1.Cl[S:10](=[O:11])(=[O:12])[c:13]1[s:14][c:15]2[cH:16][cH:17][c:18]([CH3:19])[cH:20][c:21]2[c:22]1[CH3:23]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([NH:9][S:10](=[O:11])(=[O:12])[c:13]2[s:14][c:15]3[cH:16][...
COC(=O)c1ccc(N)c(S(C)(=O)=O)c1.Cc1ccc2sc(S(=O)(=O)Cl)c(C)c2c1
COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(C)cc3c2C)c(S(C)(=O)=O)c1
null
null
C1CCOC1
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=S(=O)(Nc1ccccc1)c1cc2ccccc2s1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[#16;a:6]:[c:7].[NH2;D1;+0:8]-[c:9](:[c:10]):[c:11]>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[NH;D2;+0:8]-[c:9](:[c:10]):[c:11])-[c:4](:[c:5]):[#16;a:6]:[c:7]
50
[{"value": 50.0, "product": "CC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C(=O)OC)C=C2)S(=O)(=O)C)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
6
HOUR
Into 8.0 mL of THF was dissolved 183 mg of methyl 4-amino-3-methanesulfonylbenzoate, followed by addition of 96 mg of sodium hydride (oily, 60%) at 0° C. After 20 minutes of stirring at the same temperature, 250 mg of 2-chlorosulfonyl-5-methyl-3-methylbenzo[b]thiophene was added at 0° C., followed by 6 hours of stirrin...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccccc1.c1ccc2sccc2c1
HCl
C1CCOC1
null
6
COC(=O)c1ccc(N)c(S(C)(=O)=O)c1.Cc1ccc2sc(S(=O)(=O)Cl)c(C)c2c1>C1CCOC1>COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(C)cc3c2C)c(S(C)(=O)=O)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-dfaf5cab0b8e4e7188a11fb0523060d5
COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(Cl)cc3c2C)c(S(C)(=O)=O)c1>>COC(=O)c1ccc(NS(=O)(=O)c2sc3ccccc3c2C)c(S(C)(=O)=O)c1
CO.ClC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C(=O)OC)C=C2)S(=O)(=O)C)C=C1>>CC=1C2=C(SC1S(=O)(=O)NC1=C(C=C(C(=O)OC)C=C1)S(=O)(=O)C)C=CC=C2
Cl[c:18]1[cH:17][cH:16][c:15]2[s:14][c:13]([S:10]([NH:9][c:8]3[cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:28][c:23]3[S:24]([CH3:25])(=[O:26])=[O:27])(=[O:11])=[O:12])[c:21]([CH3:22])[c:20]2[cH:19]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([NH:9][S:10](=[O:11])(=[O:12])[c:13]2[s:14][c:15]3[cH:16][cH:17][cH:...
COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(Cl)cc3c2C)c(S(C)(=O)=O)c1
COC(=O)c1ccc(NS(=O)(=O)c2sc3ccccc3c2C)c(S(C)(=O)=O)c1
null
[Pd]
O1CCOCC1
Functional Group Interconversion
Aromatic dehalogenation
ab6c258853a046ce112a28199ff0524dc13007f2a0961d19b739094801efd0b3
56de34d4a44cb25d9380269ee5e138b0f24b40a3a0db22c5508049dc775a861f
O=S(=O)(Nc1ccccc1)c1cc2ccccc2s1
Cl-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](:[#16;a:5]):[c:6]:[c:7]:1>>[#16;a:5]:[c:4]1:[c:3]:[c:2]:[cH;D2;+0:1]:[c:7]:[c:6]:1
22.9
[{"value": 22.9, "product": "CC=1C2=C(SC1S(=O)(=O)NC1=C(C=C(C(=O)OC)C=C1)S(=O)(=O)C)C=CC=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
10
MINUTE
Into a mixed solvent of 30 mL of methanol and 30 mL of dioxane was dissolved 640 mg of 5% palladium/carbon, followed by 10 minutes of stirring under a hydrogen atmosphere. Under an argon atmosphere, 330 mg of Compound 1 was added, followed by 3 days of stirring under a hydrogen atmosphere at 5 atm. After confirmation o...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1ccc2sccc2c1
c1ccc2sccc2c1
c1ccccc1.c1ccc2sccc2c1
Other
[Pd].O1CCOCC1
null
0.166667
COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(Cl)cc3c2C)c(S(C)(=O)=O)c1>[Pd].O1CCOCC1>COC(=O)c1ccc(NS(=O)(=O)c2sc3ccccc3c2C)c(S(C)(=O)=O)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-9df67f8241b94f8eab40a4e21dcad1f1
COC(=O)c1coc(-c2ccc(NS(=O)(=O)c3sc4ccc(F)cc4c3C)c(S(C)(=O)=O)c2)n1>>Cc1c(S(=O)(=O)Nc2ccc(-c3nc(C(=O)O)co3)cc2S(C)(=O)=O)sc2ccc(F)cc12
CO.FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)C=2OC=C(N2)C(=O)OC)S(=O)(=O)C)C=C1.[OH-].[Na+]>>FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)C=2OC=C(N2)C(=O)O)S(=O)(=O)C)C=C1
C[O:17][C:15]([c:14]1[n:13][c:12](-[c:11]2[cH:10][cH:9][c:8]([NH:7][S:4]([c:3]3[c:2]([CH3:1])[c:33]4[c:27]([s:26]3)[cH:28][cH:29][c:30]([F:31])[cH:32]4)(=[O:5])=[O:6])[c:21]([S:22]([CH3:23])(=[O:24])=[O:25])[cH:20]2)[o:19][cH:18]1)=[O:16]>>[CH3:1][c:2]1[c:3]([S:4](=[O:5])(=[O:6])[NH:7][c:8]2[cH:9][cH:10][c:11](-[c:12]3...
COC(=O)c1coc(-c2ccc(NS(=O)(=O)c3sc4ccc(F)cc4c3C)c(S(C)(=O)=O)c2)n1
Cc1c(S(=O)(=O)Nc2ccc(-c3nc(C(=O)O)co3)cc2S(C)(=O)=O)sc2ccc(F)cc12
null
null
O
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=S(=O)(Nc1ccc(-c2ncco2)cc1)c1cc2ccccc2s1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4](:[#7;a:5]):[c:6]:[#8;a:7]>>[#7;a:5]:[c:4](-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]):[c:6]:[#8;a:7]
75.7
[{"value": 75.7, "product": "FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)C=2OC=C(N2)C(=O)O)S(=O)(=O)C)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
Into 150 mL of methanol was dissolved 7.85 g of Compound 23, and 15 mL of 10% aqueous sodium hydroxide solution and 15 mL of water were added thereto at room temperature, followed by 15 minutes of stirring. The precipitated crystals were dissolved by adding 90 mL of water, and the solution was stirred at the same tempe...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1cocn1.c1ccc2sccc2c1
Other
O
null
0.25
COC(=O)c1coc(-c2ccc(NS(=O)(=O)c3sc4ccc(F)cc4c3C)c(S(C)(=O)=O)c2)n1>O>Cc1c(S(=O)(=O)Nc2ccc(-c3nc(C(=O)O)co3)cc2S(C)(=O)=O)sc2ccc(F)cc12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-89c4ff77a58446e3918a1698969d9ac0
CO.COC(=O)c1coc(-c2ccc(NS(=O)(=O)c3sc4ccc(F)cc4c3C)c(S(C)(=O)=O)c2)n1.C[O-]>>Cc1c(S(=O)(=O)Nc2ccc(-c3nc(C(=O)[O-])co3)cc2S(C)(=O)=O)sc2ccc(F)cc12.Cc1c(S(=O)(=O)Nc2ccc(-c3nc(C(=O)[O-])co3)cc2S(C)(=O)=O)sc2ccc(F)cc12.[Na+]
CO.FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)C=2OC=C(N2)C(=O)OC)S(=O)(=O)C)C=C1.C[O-].[Na+]>>FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)C=2OC=C(N2)C(=O)[O-])S(=O)(=O)C)C=C1.[Na+].[Na+].FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)C=2OC=C(N2)C(=O)[O-])S(=O)(=O)C)C=C1
[CH3:36][OH:50].[CH3:1][c:2]1[c:3]([S:4](=[O:5])([NH:7][c:8]2[cH:9][cH:10][c:11](-[c:12]3[n:13][c:14]([C:15](=[O:16])[O:17][CH3:34])[cH:18][o:19]3)[cH:20][c:21]2[S:22]([CH3:23])(=[O:24])=[O:25])=[O:58])[s:26][c:27]2[cH:28][cH:29][c:30]([F:31])[cH:32][c:33]12.[O-:52][CH3:65]>>[CH3:1][c:2]1[c:3]([S:4](=[O:5])(=[O:6])[NH:...
CO.COC(=O)c1coc(-c2ccc(NS(=O)(=O)c3sc4ccc(F)cc4c3C)c(S(C)(=O)=O)c2)n1.C[O-]
Cc1c(S(=O)(=O)Nc2ccc(-c3nc(C(=O)[O-])co3)cc2S(C)(=O)=O)sc2ccc(F)cc12.Cc1c(S(=O)(=O)Nc2ccc(-c3nc(C(=O)[O-])co3)cc2S(C)(=O)=O)sc2ccc(F)cc12.[Na+]
null
null
CCOCC
Aromatic Heterocycle Formation
OtherReaction
26022037f8d7c84b958e14966f0bcd76e966ebf215529d8ad30dc9f8d5064d07
cd1d61d325f3072edfb3fd370ba9e4b1a70ae92ebeaf5ee47d1c354d420de8de
O=S(=O)(Nc1ccc(-c2ncco2)cc1)c1cc2ccccc2s1.O=S(=O)(Nc1ccc(-c2ncco2)cc1)c1cc2ccccc2s1
[#7;a:1]:[c:2](-[C:3](=[O;D1;H0:4])-[O;H0;D2;+0:5]-[CH3;D1;+0:6]):[c:7]:[#8;a:8].[O;D1;H0:9]=[S;H0;D4;+0:10](=[O;H0;D1;+0:11])(-[#7:12]-[c:13])-[c:14](:[c:15]):[#16;a:16]:[c:17].[CH3;D1;+0:18]-[O-;H0;D1:19].[CH3;D1;+0:20]-[OH;D1;+0:21]>>[#7;a:1]:[c:2](-[C:3](-[O-;H0;D1:5])=[O;D1;H0:4]):[c:7]:[#8;a:8].[O;D1;H0:9]=[S;H0;...
101.9
[{"value": 101.9, "product": "FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)C=2OC=C(N2)C(=O)[O-])S(=O)(=O)C)C=C1.[Na+].[Na+].FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)C=2OC=C(N2)C(=O)[O-])S(=O)(=O)C)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
Into 30 mL of methanol was dissolved 290 mg of Compound 23, followed by addition of 77 mg of sodium methoxide. After 8 hours of stirring at room temperature, ether was added and the precipitated crystals were collected by filtration and washed with ether to obtain 300 mg of the title compound as colorless powder. Condi...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Ester.Methanol
Sulfonamide.Sulfonamide.Aromatic halide.Sulfone
null
c1ccccc1.c1cocn1.c1ccc2sccc2c1
c1ccccc1.c1cocn1.c1ccc2sccc2c1.c1ccccc1.c1cocn1.c1ccc2sccc2c1
null
CCOCC
null
8
CO.COC(=O)c1coc(-c2ccc(NS(=O)(=O)c3sc4ccc(F)cc4c3C)c(S(C)(=O)=O)c2)n1.C[O-]>CCOCC>Cc1c(S(=O)(=O)Nc2ccc(-c3nc(C(=O)[O-])co3)cc2S(C)(=O)=O)sc2ccc(F)cc12.Cc1c(S(=O)(=O)Nc2ccc(-c3nc(C(=O)[O-])co3)cc2S(C)(=O)=O)sc2ccc(F)cc12.[Na+]
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-506f97002f0944aab9bd2fc61fbd9358
COc1sc(-c2ccc(N)c(S(C)(=O)=O)c2)nc1C.Cc1c(S(=O)(=O)Cl)sc2ccc(F)cc12>>COc1sc(-c2ccc(NS(=O)(=O)c3sc4ccc(F)cc4c3C)c(S(C)(=O)=O)c2)nc1C
Cl.ClS(=O)(=O)C1=C(C2=C(S1)C=CC(=C2)F)C.[H-].[Na+].CS(=O)(=O)C1=C(N)C=CC(=C1)C=1SC(=C(N1)C)OC>>FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)C=2SC(=C(N2)C)OC)S(=O)(=O)C)C=C1
[CH3:1][O:2][c:3]1[s:4][c:5](-[c:6]2[cH:7][cH:8][c:9]([NH2:10])[c:25]([S:26]([CH3:27])(=[O:28])=[O:29])[cH:30]2)[n:31][c:32]1[CH3:33].Cl[S:11](=[O:12])(=[O:13])[c:14]1[s:15][c:16]2[cH:17][cH:18][c:19]([F:20])[cH:21][c:22]2[c:23]1[CH3:24]>>[CH3:1][O:2][c:3]1[s:4][c:5](-[c:6]2[cH:7][cH:8][c:9]([NH:10][S:11](=[O:12])(=[O:...
COc1sc(-c2ccc(N)c(S(C)(=O)=O)c2)nc1C.Cc1c(S(=O)(=O)Cl)sc2ccc(F)cc12
COc1sc(-c2ccc(NS(=O)(=O)c3sc4ccc(F)cc4c3C)c(S(C)(=O)=O)c2)nc1C
null
null
CC(=O)N(C)C.C1CCOC1
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=S(=O)(Nc1ccc(-c2nccs2)cc1)c1cc2ccccc2s1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[#16;a:6]:[c:7].[NH2;D1;+0:8]-[c:9](:[c:10]):[c:11]>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[NH;D2;+0:8]-[c:9](:[c:10]):[c:11])-[c:4](:[c:5]):[#16;a:6]:[c:7]
70.5
[{"value": 70.5, "product": "FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)C=2SC(=C(N2)C)OC)S(=O)(=O)C)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-25
CELSIUS
10
MINUTE
Under an argon atmosphere, 41 mg of 2-methanesulfonyl-4-(5-methoxy-4-methylthiazol-2-yl)aniline was dissolved into a mixed solution of 3 mL of THF and 3 mL of dimethylacetamide. The solution was cooled to −25° C. and 15 mg of sodium hydride (oily, 60%) was added thereto, followed by 10 minutes of stirring at the same t...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1cscn1.c1ccccc1.c1ccc2sccc2c1
HCl
CC(=O)N(C)C.C1CCOC1
-25
0.166667
COc1sc(-c2ccc(N)c(S(C)(=O)=O)c2)nc1C.Cc1c(S(=O)(=O)Cl)sc2ccc(F)cc12>CC(=O)N(C)C.C1CCOC1>COc1sc(-c2ccc(NS(=O)(=O)c3sc4ccc(F)cc4c3C)c(S(C)(=O)=O)c2)nc1C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-9673436fbafd4e999edf685887af37da
CC(=O)CNC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(F)cc3c2C)c(S(C)(=O)=O)c1.S=P12SP3(=S)SP(=S)(S1)SP(=S)(S2)S3>>Cc1cnc(-c2ccc(NS(=O)(=O)c3sc4ccc(F)cc4c3C)c(S(C)(=O)=O)c2)s1
FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C(=O)NCC(C)=O)C=C2)S(=O)(=O)C)C=C1.P12(=S)SP3(=S)SP(=S)(S1)SP(=S)(S2)S3>>FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)C=2SC(=CN2)C)S(=O)(=O)C)C=C1
O=[C:2]([CH3:1])[CH2:3][NH:4][C:5](=O)[c:6]1[cH:7][cH:8][c:9]([NH:10][S:11](=[O:12])(=[O:13])[c:14]2[s:15][c:16]3[cH:17][cH:18][c:19]([F:20])[cH:21][c:22]3[c:23]2[CH3:24])[c:25]([S:26]([CH3:27])(=[O:28])=[O:29])[cH:30]1.S=P12SP3(=S)SP(=S)(S1)[S:31]P(=S)(S2)S3>>[CH3:1][c:2]1[cH:3][n:4][c:5](-[c:6]2[cH:7][cH:8][c:9]([NH:...
CC(=O)CNC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(F)cc3c2C)c(S(C)(=O)=O)c1.S=P12SP3(=S)SP(=S)(S1)SP(=S)(S2)S3
Cc1cnc(-c2ccc(NS(=O)(=O)c3sc4ccc(F)cc4c3C)c(S(C)(=O)=O)c2)s1
null
null
O1CCOCC1
Miscellaneous
OtherReaction
a308741a740680bec166bc8e57be6165194b01af60efe4a9b838a9dd9812f89a
fc147a74b43bd8ea0c955e2e68acca90d32ef33bb23f18686fa46c093607a24f
O=S(=O)(Nc1ccc(-c2nccs2)cc1)c1cc2ccccc2s1
O=[C;H0;D3;+0:1](-[C;D1;H3:2])-[CH2;D2;+0:3]-[NH;D2;+0:4]-[C;H0;D3;+0:5](=O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10].S=P12-S-P3(=S)-S-P(=S)(-S-1)-[S;H0;D2;+0:11]-P(=S)(-S-2)-S-3>>[C;D1;H3:2]-[c;H0;D3;+0:1]1:[cH;D2;+0:3]:[n;H0;D2;+0:4]:[c;H0;D3;+0:5](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[s;H0;D2;+0:11]:1
77
[{"value": 77.0, "product": "FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)C=2SC(=CN2)C)S(=O)(=O)C)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
4.5
HOUR
Into 5 mL of 1,4-dioxane solution of 150 mg of 4-(5-fluoro-3-methylbenzo[b]thiophene-2-yl)sulfonamido-3-methanesulfonyl-N-(2-oxopropyl)benzamide was added 135 mg of diphosphorus pentasulfide, followed by 4.5 hours of heating under refluxing. The reaction was terminated by adding water to the reaction mixture and the mi...
10.6084/m9.figshare.5104873.v1
null
Ketone.Secondary amide.Monosulfide.Monosulfide.Monosulfide.Monosulfide.Monosulfide.Monosulfide
null
S1P2SP3SP1SP(S2)S3
c1cscn1
c1cscn1.c1ccccc1.c1ccc2sccc2c1
Other
O1CCOCC1
null
4.5
CC(=O)CNC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(F)cc3c2C)c(S(C)(=O)=O)c1.S=P12SP3(=S)SP(=S)(S1)SP(=S)(S2)S3>O1CCOCC1>Cc1cnc(-c2ccc(NS(=O)(=O)c3sc4ccc(F)cc4c3C)c(S(C)(=O)=O)c2)s1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-8d1b90adae4349a2acadac9aa9c5d382
Cc1c(S(=O)(=O)Nc2ccc(-c3nc(CO)cs3)cc2S(C)(=O)=O)sc2ccc(F)cc12.O=S(Cl)Cl>>Cc1c(S(=O)(=O)Nc2ccc(-c3nc(CCl)cs3)cc2S(C)(=O)=O)sc2ccc(F)cc12
S(=O)(Cl)Cl.C(Cl)(Cl)Cl.FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)C=2SC=C(N2)CO)S(=O)(=O)C)C=C1.S(=O)(Cl)Cl>>ClCC=1N=C(SC1)C1=CC(=C(C=C1)NS(=O)(=O)C1=C(C2=C(S1)C=CC(=C2)F)C)S(=O)(=O)C
O[CH2:15][c:14]1[n:13][c:12](-[c:11]2[cH:10][cH:9][c:8]([NH:7][S:4]([c:3]3[c:2]([CH3:1])[c:32]4[c:26]([s:25]3)[cH:27][cH:28][c:29]([F:30])[cH:31]4)(=[O:5])=[O:6])[c:20]([S:21]([CH3:22])(=[O:23])=[O:24])[cH:19]2)[s:18][cH:17]1.O=S(Cl)[Cl:16]>>[CH3:1][c:2]1[c:3]([S:4](=[O:5])(=[O:6])[NH:7][c:8]2[cH:9][cH:10][c:11](-[c:12...
Cc1c(S(=O)(=O)Nc2ccc(-c3nc(CO)cs3)cc2S(C)(=O)=O)sc2ccc(F)cc12.O=S(Cl)Cl
Cc1c(S(=O)(=O)Nc2ccc(-c3nc(CCl)cs3)cc2S(C)(=O)=O)sc2ccc(F)cc12
null
null
C(C)N(CC)CC
Functional Group Interconversion
Alcohol to chloride_SOCl2
bb752b9027dc4488ba075e5955118a819f80cabd751a7497b67c2eeb1db6b071
cbf41c7cf9fe6b47a243b1674d74ed5bf46a151f7f3a71d206e23176e158facf
O=S(=O)(Nc1ccc(-c2nccs2)cc1)c1cc2ccccc2s1
Cl-S(=O)-[Cl;H0;D1;+0:1].O-[CH2;D2;+0:2]-[c:3]1:[#7;a:4]:[c:5]:[#16;a:6]:[c:7]:1>>[Cl;H0;D1;+0:1]-[CH2;D2;+0:2]-[c:3]1:[#7;a:4]:[c:5]:[#16;a:6]:[c:7]:1
null
[]
null
null
21
HOUR
Into 20 mL of chloroform was suspended 159 mg of Compound 63, and 47 μL of thionyl chloride was added at 0° C., followed by 21 hours of stirring at room temperature. Further, 1 mL of thionyl chloride was added, followed by 1 hour of heating under refluxing. After 2 mL of triethylamine was added at 0° C. and the mixture...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Primary halide
null
null
c1ccccc1.c1cscn1.c1ccc2sccc2c1
HCl
C(C)N(CC)CC
null
21
Cc1c(S(=O)(=O)Nc2ccc(-c3nc(CO)cs3)cc2S(C)(=O)=O)sc2ccc(F)cc12.O=S(Cl)Cl>C(C)N(CC)CC>Cc1c(S(=O)(=O)Nc2ccc(-c3nc(CCl)cs3)cc2S(C)(=O)=O)sc2ccc(F)cc12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-41efe53e0c8b4b2eb8ad50e1253946aa
Cc1c(S(=O)(=O)Nc2ccc(-c3nc(CCl)cs3)cc2S(C)(=O)=O)sc2ccc(F)cc12>>Cc1csc(-c2ccc(NS(=O)(=O)c3sc4ccc(F)cc4c3C)c(S(C)(=O)=O)c2)n1
ClCC=1N=C(SC1)C1=CC(=C(C=C1)NS(=O)(=O)C1=C(C2=C(S1)C=CC(=C2)F)C)S(=O)(=O)C.[I-].[Na+].[I-].[Na+]>>FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)C=2SC=C(N2)C)S(=O)(=O)C)C=C1
Cl[CH2:1][c:2]1[cH:3][s:4][c:5](-[c:6]2[cH:7][cH:8][c:9]([NH:10][S:11](=[O:12])(=[O:13])[c:14]3[s:15][c:16]4[cH:17][cH:18][c:19]([F:20])[cH:21][c:22]4[c:23]3[CH3:24])[c:25]([S:26]([CH3:27])(=[O:28])=[O:29])[cH:30]2)[n:31]1>>[CH3:1][c:2]1[cH:3][s:4][c:5](-[c:6]2[cH:7][cH:8][c:9]([NH:10][S:11](=[O:12])(=[O:13])[c:14]3[s:...
Cc1c(S(=O)(=O)Nc2ccc(-c3nc(CCl)cs3)cc2S(C)(=O)=O)sc2ccc(F)cc12
Cc1csc(-c2ccc(NS(=O)(=O)c3sc4ccc(F)cc4c3C)c(S(C)(=O)=O)c2)n1
null
null
CC(=O)C
Functional Group Interconversion
Dehalogenation
72a5231b07f184f0ef4a0648badd4176f521b95f1ba3340a0f90d8894af47260
47a659f5704a5b7ca1b92ff731f18f109c6bde1d45152a3a393eefbd10265508
O=S(=O)(Nc1ccc(-c2nccs2)cc1)c1cc2ccccc2s1
Cl-[CH2;D2;+0:1]-[c:2]1:[#7;a:3]:[c:4]:[#16;a:5]:[c:6]:1>>[CH3;D1;+0:1]-[c:2]1:[#7;a:3]:[c:4]:[#16;a:5]:[c:6]:1
48.5
[{"value": 48.5, "product": "FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)C=2SC=C(N2)C)S(=O)(=O)C)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
24
HOUR
Into 10 mL of acetone was dissolved 64 mg of Compound 64, and 180 mg of sodium iodide was added, followed by 24 hours of heating under refluxing. Further, 180 mg of sodium iodide was added and the mixture was heated under refluxing for 19 hours. The solvent was removed by evaporation under reduced pressure and the resi...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
null
null
c1cscn1.c1ccccc1.c1ccc2sccc2c1
Other
CC(=O)C
null
24
Cc1c(S(=O)(=O)Nc2ccc(-c3nc(CCl)cs3)cc2S(C)(=O)=O)sc2ccc(F)cc12>CC(=O)C>Cc1csc(-c2ccc(NS(=O)(=O)c3sc4ccc(F)cc4c3C)c(S(C)(=O)=O)c2)n1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f731784ee373406e9c581e111ac0c2f4
COC(=O)c1csc(-c2ccc(NS(=O)(=O)c3sc4ccc(F)cc4c3C)c(S(C)(=O)=O)c2)n1>>Cc1c(S(=O)(=O)Nc2ccc(-c3nc(C(=O)O)cs3)cc2S(C)(=O)=O)sc2ccc(F)cc12
FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)C=2SC=C(N2)C(=O)OC)S(=O)(=O)C)C=C1.[OH-].[Na+]>>FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)C=2SC=C(N2)C(=O)O)S(=O)(=O)C)C=C1
C[O:17][C:15]([c:14]1[n:13][c:12](-[c:11]2[cH:10][cH:9][c:8]([NH:7][S:4]([c:3]3[c:2]([CH3:1])[c:33]4[c:27]([s:26]3)[cH:28][cH:29][c:30]([F:31])[cH:32]4)(=[O:5])=[O:6])[c:21]([S:22]([CH3:23])(=[O:24])=[O:25])[cH:20]2)[s:19][cH:18]1)=[O:16]>>[CH3:1][c:2]1[c:3]([S:4](=[O:5])(=[O:6])[NH:7][c:8]2[cH:9][cH:10][c:11](-[c:12]3...
COC(=O)c1csc(-c2ccc(NS(=O)(=O)c3sc4ccc(F)cc4c3C)c(S(C)(=O)=O)c2)n1
Cc1c(S(=O)(=O)Nc2ccc(-c3nc(C(=O)O)cs3)cc2S(C)(=O)=O)sc2ccc(F)cc12
null
null
CO
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=S(=O)(Nc1ccc(-c2nccs2)cc1)c1cc2ccccc2s1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4](:[#7;a:5]):[c:6]:[#16;a:7]>>[#16;a:7]:[c:6]:[c:4](-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]):[#7;a:5]
80.3
[{"value": 80.3, "product": "FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)C=2SC=C(N2)C(=O)O)S(=O)(=O)C)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
20
MINUTE
Into 45 mL of methanol was dissolved 954 mg of Compound 69, and 4.0 mL of 1 mol/L sodium hydroxide was added thereto. After 20 minutes of stirring under heating and refluxing, the solvent was removed by evaporation under reduced pressure, and the resulting residue was extracted with ether-water (1/1). To the aqueous la...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1cscn1.c1ccc2sccc2c1
Other
CO
null
0.333333
COC(=O)c1csc(-c2ccc(NS(=O)(=O)c3sc4ccc(F)cc4c3C)c(S(C)(=O)=O)c2)n1>CO>Cc1c(S(=O)(=O)Nc2ccc(-c3nc(C(=O)O)cs3)cc2S(C)(=O)=O)sc2ccc(F)cc12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4e4aa71acf48406f8e6045f64380a89b
CC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(F)cc3c2C)c(S(C)(=O)=O)c1.[Br-]>>Cc1c(S(=O)(=O)Nc2ccc(C(=O)CBr)cc2S(C)(=O)=O)sc2ccc(F)cc12
C(C)(=O)C1=CC(=C(C=C1)NS(=O)(=O)C1=C(C2=C(S1)C=CC(=C2)F)C)S(=O)(=O)C.[Br-].[Br-].[Br-].C(C1=CC=CC=C1)[N+](C)(C)C.C(C1=CC=CC=C1)[N+](C)(C)C.C(C1=CC=CC=C1)[N+](C)(C)C>>BrCC(=O)C1=CC(=C(C=C1)NS(=O)(=O)C1=C(C2=C(S1)C=CC(=C2)F)C)S(=O)(=O)C
[CH3:1][c:2]1[c:3]([S:4](=[O:5])(=[O:6])[NH:7][c:8]2[cH:9][cH:10][c:11]([C:12](=[O:13])[CH3:14])[cH:16][c:17]2[S:18]([CH3:19])(=[O:20])=[O:21])[s:22][c:23]2[cH:24][cH:25][c:26]([F:27])[cH:28][c:29]12.[Br-:15]>>[CH3:1][c:2]1[c:3]([S:4](=[O:5])(=[O:6])[NH:7][c:8]2[cH:9][cH:10][c:11]([C:12](=[O:13])[CH2:14][Br:15])[cH:16]...
CC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(F)cc3c2C)c(S(C)(=O)=O)c1.[Br-]
Cc1c(S(=O)(=O)Nc2ccc(C(=O)CBr)cc2S(C)(=O)=O)sc2ccc(F)cc12
null
null
C(Cl)(Cl)Cl
Functional Group Interconversion
Bromination
97ca6720945af5a02c450d33ec56e946521050f9771c27f9cfcb85f3477593f6
cb3e14519230141aa015a4cf9c960def3e60f01997e61621f62506924bfa15de
O=S(=O)(Nc1ccccc1)c1cc2ccccc2s1
[Br-;H0;D0:1].[CH3;D1;+0:2]-[C:3](=[O;D1;H0:4])-[c:5]>>[Br;H0;D1;+0:1]-[CH2;D2;+0:2]-[C:3](=[O;D1;H0:4])-[c:5]
137.5
[{"value": 137.5, "product": "BrCC(=O)C1=CC(=C(C=C1)NS(=O)(=O)C1=C(C2=C(S1)C=CC(=C2)F)C)S(=O)(=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
Into 4.0 mL of chloroform was dissolved 200 mg of Compound 19, and 194 mg of benzyltrimethylammonium tribromide was added, followed by 1 hour of stirring at room temperature. The reaction was terminated by adding water to the reaction solution and then the solvent was once removed by evaporation. The residue was adjust...
10.6084/m9.figshare.5104873.v1
null
Ketone
Primary halide
null
null
c1ccccc1.c1ccc2sccc2c1
null
C(Cl)(Cl)Cl
null
1
CC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(F)cc3c2C)c(S(C)(=O)=O)c1.[Br-]>C(Cl)(Cl)Cl>Cc1c(S(=O)(=O)Nc2ccc(C(=O)CBr)cc2S(C)(=O)=O)sc2ccc(F)cc12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b7c1db2cb9ec4c41b044969a894ab304
CC(N)=S.Cc1c(S(=O)(=O)Nc2ccc(C(=O)CBr)cc2S(C)(=O)=O)sc2ccc(F)cc12>>Cc1nc(-c2ccc(NS(=O)(=O)c3sc4ccc(F)cc4c3C)c(S(C)(=O)=O)c2)cs1
BrCC(=O)C1=CC(=C(C=C1)NS(=O)(=O)C1=C(C2=C(S1)C=CC(=C2)F)C)S(=O)(=O)C.O1CCOCC1.C(O)([O-])=O.[Na+].C(C)(=S)N>>FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)C=2N=C(SC2)C)S(=O)(=O)C)C=C1
[CH3:1][C:2]([NH2:3])=[S:31].O=[C:4]([c:5]1[cH:6][cH:7][c:8]([NH:9][S:10](=[O:11])(=[O:12])[c:13]2[s:14][c:15]3[cH:16][cH:17][c:18]([F:19])[cH:20][c:21]3[c:22]2[CH3:23])[c:24]([S:25]([CH3:26])(=[O:27])=[O:28])[cH:29]1)[CH2:30]Br>>[CH3:1][c:2]1[n:3][c:4](-[c:5]2[cH:6][cH:7][c:8]([NH:9][S:10](=[O:11])(=[O:12])[c:13]3[s:1...
CC(N)=S.Cc1c(S(=O)(=O)Nc2ccc(C(=O)CBr)cc2S(C)(=O)=O)sc2ccc(F)cc12
Cc1nc(-c2ccc(NS(=O)(=O)c3sc4ccc(F)cc4c3C)c(S(C)(=O)=O)c2)cs1
null
null
C(C)O
Aromatic Heterocycle Formation
OtherReaction
21eb8c7cda3c7fc14309a0c556334226f1a9147c334386d33bc70341830a82ec
9f145257a80f08f1a7a6ee36c84cd4115965bd63128f36de61c7ed688ad2603c
O=S(=O)(Nc1ccc(-c2cscn2)cc1)c1cc2ccccc2s1
Br-[CH2;D2;+0:1]-[C;H0;D3;+0:2](=O)-[c;H0;D3;+0:3](:[c:4]:[c:5]):[c:6]:[c:7].[C;D1;H3:8]-[C;H0;D3;+0:9](-[NH2;D1;+0:10])=[S;H0;D1;+0:11]>>[C;D1;H3:8]-[c;H0;D3;+0:9]1:[n;H0;D2;+0:10]:[c;H0;D3;+0:2](-[c;H0;D3;+0:3](:[c:4]:[c:5]):[c:6]:[c:7]):[cH;D2;+0:1]:[s;H0;D2;+0:11]:1
42.6
[{"value": 42.6, "product": "FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)C=2N=C(SC2)C)S(=O)(=O)C)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
Into 4.0 mL of chloroform was dissolved 200 mg of Compound 19, and 194 mg of benzyltrimethylammonium tribromide was added, followed by 1 hour of stirring at room temperature. The reaction was terminated by adding water to the reaction solution and then the solvent was once removed by evaporation. The residue was adjust...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ketone.Thioamide
null
null
c1cscn1
c1cscn1.c1ccccc1.c1ccc2sccc2c1
HBr
C(C)O
null
2
CC(N)=S.Cc1c(S(=O)(=O)Nc2ccc(C(=O)CBr)cc2S(C)(=O)=O)sc2ccc(F)cc12>C(C)O>Cc1nc(-c2ccc(NS(=O)(=O)c3sc4ccc(F)cc4c3C)c(S(C)(=O)=O)c2)cs1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ff5388fdf5e343ff9a10e18ce76848f7
COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(F)cc3c2C)c(S(C)(=O)=O)c1>>Cc1c(S(=O)(=O)Nc2ccc(CO)cc2S(C)(=O)=O)sc2ccc(F)cc12
C(=O)([O-])C(O)C(O)C(=O)[O-].[Na+].[K+].C1(=CC=CC=C1)C.FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C(=O)OC)C=C2)S(=O)(=O)C)C=C1.C1(=CC=CC=C1)C.[H-].C(C(C)C)[Al+]CC(C)C>>FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)CO)S(=O)(=O)C)C=C1
CO[C:12]([c:11]1[cH:10][cH:9][c:8]([NH:7][S:4]([c:3]2[c:2]([CH3:1])[c:27]3[c:21]([s:20]2)[cH:22][cH:23][c:24]([F:25])[cH:26]3)(=[O:5])=[O:6])[c:15]([S:16]([CH3:17])(=[O:18])=[O:19])[cH:14]1)=[O:13]>>[CH3:1][c:2]1[c:3]([S:4](=[O:5])(=[O:6])[NH:7][c:8]2[cH:9][cH:10][c:11]([CH2:12][OH:13])[cH:14][c:15]2[S:16]([CH3:17])(=[...
COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(F)cc3c2C)c(S(C)(=O)=O)c1
Cc1c(S(=O)(=O)Nc2ccc(CO)cc2S(C)(=O)=O)sc2ccc(F)cc12
null
null
O.C(C)(=O)OCC
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
O=S(=O)(Nc1ccccc1)c1cc2ccccc2s1
C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3](:[c:4]):[c:5]>>[OH;D1;+0:2]-[CH2;D2;+0:1]-[c:3](:[c:4]):[c:5]
70.7
[{"value": 70.7, "product": "FC1=CC2=C(SC(=C2C)S(=O)(=O)NC2=C(C=C(C=C2)CO)S(=O)(=O)C)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-30
CELSIUS
null
null
Into 120 mL of toluene was dissolved 2.08 g of Compound 17. After cooling to −30° C., 22.5 mL of 1.01 mol/L toluene solution of diisobutylaluminum hydride was added thereto. After 5 hours of stirring at the same temperature, water was added to the reaction solution to terminate the reaction and then the mixture was dil...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
c1ccccc1.c1ccc2sccc2c1
Other
O.C(C)(=O)OCC
-30
null
COC(=O)c1ccc(NS(=O)(=O)c2sc3ccc(F)cc3c2C)c(S(C)(=O)=O)c1>O.C(C)(=O)OCC>Cc1c(S(=O)(=O)Nc2ccc(CO)cc2S(C)(=O)=O)sc2ccc(F)cc12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-556fc30c333c40f3bdcee69717499612
CCOC(C(=O)OC)P(=O)(OCC)OCC.O=Cc1ccc(OCCCl)cc1>>CCOC(=Cc1ccc(OCCCl)cc1)C(=O)OC
[H-].[Na+].C(C)OC(C(=O)OC)P(=O)(OCC)OCC.ClCCOC1=CC=C(C=O)C=C1>>ClCCOC1=CC=C(C=C1)C=C(C(=O)OC)OCC
CCOP(=O)(OCC)[CH:4]([O:3][CH2:2][CH3:1])[C:16](=[O:17])[O:18][CH3:19].O=[CH:5][c:6]1[cH:7][cH:8][c:9]([O:10][CH2:11][CH2:12][Cl:13])[cH:14][cH:15]1>>[CH3:1][CH2:2][O:3][C:4](=[CH:5][c:6]1[cH:7][cH:8][c:9]([O:10][CH2:11][CH2:12][Cl:13])[cH:14][cH:15]1)[C:16](=[O:17])[O:18][CH3:19]
CCOC(C(=O)OC)P(=O)(OCC)OCC.O=Cc1ccc(OCCCl)cc1
CCOC(=Cc1ccc(OCCCl)cc1)C(=O)OC
null
null
O1CCCC1
C-C Coupling
OtherReaction
8652fada27b05b79779ff34a157bb972c7cd6d780fd24e805781fdaca3689897
ad62a0adadbf9069bf98289a96ce8b021437ecd0412624495fbcba2ade6d16f3
c1ccccc1
C-C-O-P(=O)(-O-C-C)-[CH;D3;+0:1](-[#8:2]-[C:3])-[C:4](=[O;D1;H0:5])-[#8:6]-[C;D1;H3:7].O=[CH;D2;+0:8]-[c:9](:[c:10]):[c:11]>>[C:3]-[#8:2]-[C;H0;D3;+0:1](=[CH;D2;+0:8]-[c:9](:[c:10]):[c:11])-[C:4](=[O;D1;H0:5])-[#8:6]-[C;D1;H3:7]
null
[]
null
null
1
HOUR
To 150 ml of freshly distilled tetrahydrofuran, placed in a bath of ice-cold water at 0° C., under argon, add sodium hydride (0.0473 mol) and then methyl 2-ethoxy-2-diethylphosphonoacetate (0.0394 mol) while maintaining the temperature at 0° C. After stirring for 1 hour, add 4-(2-chloroethoxy)benzaldehyde (0.0394 mol) ...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Ester.Ether
Ester.Ether
null
null
c1ccccc1
HO-
O1CCCC1
null
1
CCOC(C(=O)OC)P(=O)(OCC)OCC.O=Cc1ccc(OCCCl)cc1>O1CCCC1>CCOC(=Cc1ccc(OCCCl)cc1)C(=O)OC
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-7b19f6cc62aa46e2873a435775cda091
CCOC(=Cc1ccc(OCCCl)cc1)C(=O)OC>>CCOC(Cc1ccc(OCCCl)cc1)C(=O)OC
ClCCOC1=CC=C(C=C1)C=C(C(=O)OC)OCC>>ClCCOC1=CC=C(C=C1)CC(C(=O)OC)OCC
[CH3:1][CH2:2][O:3][C:4](=[CH:5][c:6]1[cH:7][cH:8][c:9]([O:10][CH2:11][CH2:12][Cl:13])[cH:14][cH:15]1)[C:16](=[O:17])[O:18][CH3:19]>>[CH3:1][CH2:2][O:3][CH:4]([CH2:5][c:6]1[cH:7][cH:8][c:9]([O:10][CH2:11][CH2:12][Cl:13])[cH:14][cH:15]1)[C:16](=[O:17])[O:18][CH3:19]
CCOC(=Cc1ccc(OCCCl)cc1)C(=O)OC
CCOC(Cc1ccc(OCCCl)cc1)C(=O)OC
null
[Pd]
O1CCCC1
Reduction
Hydrogenation (double to single)
d0e0332973c77aabb8c3717dddd351d2250737d1acb0f694289dece8c206d06e
fc479563bf5f932f09579579b5e31753bf159d03a224d56dc67a29b9e37b0ad6
c1ccccc1
[C:1]-[#8:2]-[C;H0;D3;+0:3](=[CH;D2;+0:4]-[c:5](:[c:6]):[c:7])-[C:8](=[O;D1;H0:9])-[#8:10]-[C;D1;H3:11]>>[C:1]-[#8:2]-[CH;D3;+0:3](-[CH2;D2;+0:4]-[c:5](:[c:6]):[c:7])-[C:8](=[O;D1;H0:9])-[#8:10]-[C;D1;H3:11]
null
[]
null
null
1
DAY
To 100 ml of tetrahydrofuran add the compound obtained in Step A (0.0175 mol) and then palladium-on-carbon (0.2 g). Stir at ambient temperature under hydrogen for 1 day. Filter off the palladium-on-carbon and then evaporate the filtrate. The oily product is purified on a column of silica gel using the eluant mixture: p...
10.6084/m9.figshare.5104873.v1
null
Ester.Ether
Ester.Ether
null
null
c1ccccc1
null
[Pd].O1CCCC1
null
24
CCOC(=Cc1ccc(OCCCl)cc1)C(=O)OC>[Pd].O1CCCC1>CCOC(Cc1ccc(OCCCl)cc1)C(=O)OC
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-18b711fee87f4c259f9e62bbac53b196
CCOC(Cc1ccc(OCCCl)cc1)C(=O)OC.O=C(c1ccccc1)c1ccc2c(c1)S(=O)C=N2>>CCOC(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)C(=O)OC
C(C1=CC=CC=C1)(=O)C1=CC2=C(N=CS2=O)C=C1.C([O-])([O-])=O.[K+].[K+].ClCCOC1=CC=C(C=C1)CC(C(=O)OC)OCC>>C(C1=CC=CC=C1)(=O)C1=CC2=C(N(C(S2)=O)CCOC2=CC=C(C=C2)CC(C(=O)OC)OCC)C=C1
Cl[CH2:12][CH2:11][O:10][c:9]1[cH:8][cH:7][c:6]([CH2:5][CH:4]([O:3][CH2:2][CH3:1])[C:33](=[O:34])[O:35][CH3:36])[cH:32][cH:31]1.[N:13]1=[CH:14][S:16](=[O:15])[c:17]2[cH:18][c:19]([C:20](=[O:21])[c:22]3[cH:23][cH:24][cH:25][cH:26][cH:27]3)[cH:28][cH:29][c:30]21>>[CH3:1][CH2:2][O:3][CH:4]([CH2:5][c:6]1[cH:7][cH:8][c:9]([...
CCOC(Cc1ccc(OCCCl)cc1)C(=O)OC.O=C(c1ccccc1)c1ccc2c(c1)S(=O)C=N2
CCOC(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)C(=O)OC
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
OtherReaction
42c83f048334b1ed148ed7afdbd743f45dba21a36b3061112c38545e7e60436d
3dcb031a7507da808ae5e1b8f13ca2c4f0152648164857a941ec9d83076e2a56
O=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccccc1
Cl-[CH2;D2;+0:1]-[C:2]-[#8:3].[O;H0;D1;+0:4]=[S;H0;D3;+0:5]1-[CH;D2;+0:6]=[N;H0;D2;+0:7]-[c:8](:[c:9]):[c:10]-1:[c:11]>>[#8:3]-[C:2]-[CH2;D2;+0:1]-[n;H0;D3;+0:7]1:[c:8](:[c:9]):[c:10](:[c:11]):[s;H0;D2;+0:5]:[c;H0;D3;+0:6]:1=[O;H0;D1;+0:4]
null
[]
100
CELSIUS
null
null
To 20 ml of dimethylformamide add potassium carbonate (0.01044 mol) and then 6-benzoylbenzothiazolinone (0.00453 mol). Heat at 100° C. for 1 hour. Add the compound obtained in Step B (0.00348 mol) and heat at 150° C. for 16 hours. Evaporate off the dimethylformamide. Take up the residue in 50 ml of water and then extra...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Sulfoxide
null
c1ccc2scnc2c1
c1ccc2scnc2c1
c1ccccc1.c1ccc2scnc2c1.c1ccccc1
HCl
CN(C=O)C
100
null
CCOC(Cc1ccc(OCCCl)cc1)C(=O)OC.O=C(c1ccccc1)c1ccc2c(c1)S(=O)C=N2>CN(C=O)C>CCOC(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)C(=O)OC
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e9e46de2e79a488992aeb4f0734723aa
CCOC(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)C(=O)OC.CON>>CCOC(Cc1ccc(OCCn2c(=O)sc3cc(C(=NOC)c4ccccc4)ccc32)cc1)C(=O)OC
C(C1=CC=CC=C1)(=O)C1=CC2=C(N(C(S2)=O)CCOC2=CC=C(C=C2)CC(C(=O)OC)OCC)C=C1.Cl.CON.N1=CC=CC=C1>>C(C)OC(C(=O)OC)CC1=CC=C(C=C1)OCCN1C(SC2=C1C=CC(=C2)C(C2=CC=CC=C2)=NOC)=O
O=[C:20]([c:19]1[cH:18][c:17]2[s:16][c:14](=[O:15])[n:13]([CH2:12][CH2:11][O:10][c:9]3[cH:8][cH:7][c:6]([CH2:5][CH:4]([O:3][CH2:2][CH3:1])[C:35](=[O:36])[O:37][CH3:38])[cH:34][cH:33]3)[c:32]2[cH:31][cH:30]1)[c:24]1[cH:25][cH:26][cH:27][cH:28][cH:29]1.[NH2:21][O:22][CH3:23]>>[CH3:1][CH2:2][O:3][CH:4]([CH2:5][c:6]1[cH:7]...
CCOC(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)C(=O)OC.CON
CCOC(Cc1ccc(OCCn2c(=O)sc3cc(C(=NOC)c4ccccc4)ccc32)cc1)C(=O)OC
null
null
CO
Heteroatom Alkylation and Arylation
OtherReaction
3d7a74a3d1c5abb5292963d4a3067f1fb8a89aead752dc9bb1d63522c4c0bd5c
6b0edeaa66853687109d0d530554f76edf36b01a8ec084e7ae9c709f0949a6b9
N=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccccc1
O=[C;H0;D3;+0:1](-[c:2](:[c:3]):[c:4]:[c:5]:[#16;a:6])-[c:7](:[c:8]):[c:9].[C;D1;H3:10]-[#8:11]-[NH2;D1;+0:12]>>[#16;a:6]:[c:5]:[c:4]:[c:2](-[C;H0;D3;+0:1](=[N;H0;D2;+0:12]-[#8:11]-[C;D1;H3:10])-[c:7](:[c:8]):[c:9]):[c:3]
null
[]
null
null
null
null
To 30 ml of methanol add the compound obtained in Step C (0.00198 mol), O-methyl-hydroxylamine hydrochloride (0.00594 mol) and pyridine (0.00594 mol). Heat at reflux for 3 hours. Evaporate to dryness. Add 100 ml of hydrochloric acid (1N) and then extract with 50 ml of dichloromethane twice. The organic phase is dried o...
10.6084/m9.figshare.5104873.v1
null
Ketone.Primary amine
null
null
null
c1ccccc1.c1ccc2scnc2c1.c1ccccc1
HO-
CO
null
null
CCOC(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)C(=O)OC.CON>CO>CCOC(Cc1ccc(OCCn2c(=O)sc3cc(C(=NOC)c4ccccc4)ccc32)cc1)C(=O)OC
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-8813f2ad16624e089fe1a0bc73d73751
CCOC(Cc1ccc(OCCCl)cc1)C(=O)OC.O=C(c1ccccc1)c1ccc2c(c1)S(=O)C=N2>>CCOC(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)C(=O)OC
C(C1=CC=CC=C1)(=O)C1=CC2=C(N=CS2=O)C=C1.C([O-])([O-])=O.[K+].[K+].ClCCOC1=CC=C(C=C1)CC(C(=O)OC)OCC>>C(C1=CC=CC=C1)(=O)C1=CC2=C(N(C(S2)=O)CCOC2=CC=C(C=C2)CC(C(=O)OC)OCC)C=C1
Cl[CH2:12][CH2:11][O:10][c:9]1[cH:8][cH:7][c:6]([CH2:5][CH:4]([O:3][CH2:2][CH3:1])[C:33](=[O:34])[O:35][CH3:36])[cH:32][cH:31]1.[N:13]1=[CH:14][S:16](=[O:15])[c:17]2[cH:18][c:19]([C:20](=[O:21])[c:22]3[cH:23][cH:24][cH:25][cH:26][cH:27]3)[cH:28][cH:29][c:30]21>>[CH3:1][CH2:2][O:3][CH:4]([CH2:5][c:6]1[cH:7][cH:8][c:9]([...
CCOC(Cc1ccc(OCCCl)cc1)C(=O)OC.O=C(c1ccccc1)c1ccc2c(c1)S(=O)C=N2
CCOC(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)C(=O)OC
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
OtherReaction
42c83f048334b1ed148ed7afdbd743f45dba21a36b3061112c38545e7e60436d
3dcb031a7507da808ae5e1b8f13ca2c4f0152648164857a941ec9d83076e2a56
O=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccccc1
Cl-[CH2;D2;+0:1]-[C:2]-[#8:3].[O;H0;D1;+0:4]=[S;H0;D3;+0:5]1-[CH;D2;+0:6]=[N;H0;D2;+0:7]-[c:8](:[c:9]):[c:10]-1:[c:11]>>[#8:3]-[C:2]-[CH2;D2;+0:1]-[n;H0;D3;+0:7]1:[c:8](:[c:9]):[c:10](:[c:11]):[s;H0;D2;+0:5]:[c;H0;D3;+0:6]:1=[O;H0;D1;+0:4]
null
[]
100
CELSIUS
null
null
To 20 ml of dimethylformamide add potassium carbonate (0.01044 mol) and then 6-benzoylbenzothiazolinone (0.00453 mol). Heat at 100° C. for 1 hour. Add the compound obtained in Step B of Example 1 (0.00348 mol) and heat at 150° C. for 16 hours. Evaporate off the dimethylformamide. Take up the residue in 50 ml of water a...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Sulfoxide
null
c1ccc2scnc2c1
c1ccc2scnc2c1
c1ccccc1.c1ccc2scnc2c1.c1ccccc1
HCl
CN(C=O)C
100
null
CCOC(Cc1ccc(OCCCl)cc1)C(=O)OC.O=C(c1ccccc1)c1ccc2c(c1)S(=O)C=N2>CN(C=O)C>CCOC(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)C(=O)OC
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-8787f5a444a64b81aa74c1046a7e90d1
COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)OC(C)(C)C.CON>>CON=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccc(CC(NC(=O)OC(C)(C)C)C(=O)OC)cc1
C(C1=CC=CC=C1)(=O)C1=CC2=C(N(C(S2)=O)CCOC2=CC=C(C=C2)CC(C(=O)OC)NC(=O)OC(C)(C)C)C=C1.CON>>C(C)(C)(C)OC(=O)NC(C(=O)OC)CC1=CC=C(C=C1)OCCN1C(SC2=C1C=CC(=C2)C(C2=CC=CC=C2)=NOC)=O
O=[C:4]([c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1)[c:11]1[cH:12][cH:13][c:14]2[c:15]([cH:16]1)[s:17][c:18](=[O:19])[n:20]2[CH2:21][CH2:22][O:23][c:24]1[cH:25][cH:26][c:27]([CH2:28][CH:29]([NH:30][C:31](=[O:32])[O:33][C:34]([CH3:35])([CH3:36])[CH3:37])[C:38](=[O:39])[O:40][CH3:41])[cH:42][cH:43]1.[CH3:1][O:2][NH2:3]>>[CH3:...
COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)OC(C)(C)C.CON
CON=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccc(CC(NC(=O)OC(C)(C)C)C(=O)OC)cc1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
3d7a74a3d1c5abb5292963d4a3067f1fb8a89aead752dc9bb1d63522c4c0bd5c
6b0edeaa66853687109d0d530554f76edf36b01a8ec084e7ae9c709f0949a6b9
N=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccccc1
O=[C;H0;D3;+0:1](-[c:2](:[c:3]):[c:4]:[c:5]:[#16;a:6])-[c:7](:[c:8]):[c:9].[C;D1;H3:10]-[#8:11]-[NH2;D1;+0:12]>>[#16;a:6]:[c:5]:[c:4]:[c:2](-[C;H0;D3;+0:1](=[N;H0;D2;+0:12]-[#8:11]-[C;D1;H3:10])-[c:7](:[c:8]):[c:9]):[c:3]
null
[]
null
null
null
null
Starting from the compound obtained in Step C, the procedure is as in Step B of Example 2, replacing the hydroxylamine by O-methylhydroxylamine. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Ketone.Primary amine
null
null
null
c1ccccc1.c1ccc2scnc2c1.c1ccccc1
HO-
null
null
null
COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)OC(C)(C)C.CON>>CON=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccc(CC(NC(=O)OC(C)(C)C)C(=O)OC)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b9097aceecf54623a7ba7ac7d11124e7
COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)OC(C)(C)C>>COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1
C(C1=CC=CC=C1)(=O)C1=CC2=C(N(C(S2)=O)CCOC2=CC=C(C=C2)CC(C(=O)OC)NC(=O)OC(C)(C)C)C=C1.FC(C(=O)O)(F)F>>FC(C(=O)O)(F)F.NC(C(=O)OC)CC1=CC=C(C=C1)OCCN1C(SC2=C1C=CC(=C2)C(C2=CC=CC=C2)=O)=O
CC(C)(C)OC(=O)[NH:6][CH:5]([C:3]([O:2][CH3:1])=[O:4])[CH2:7][c:8]1[cH:9][cH:10][c:11]([O:12][CH2:13][CH2:14][n:15]2[c:16](=[O:17])[s:18][c:19]3[cH:20][c:21]([C:22](=[O:23])[c:24]4[cH:25][cH:26][cH:27][cH:28][cH:29]4)[cH:30][cH:31][c:32]23)[cH:33][cH:34]1>>[CH3:1][O:2][C:3](=[O:4])[CH:5]([NH2:6])[CH2:7][c:8]1[cH:9][cH:1...
COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)OC(C)(C)C
COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1
null
null
ClCCl
Reduction
Hydrogenolysis of amides/imides/carbamates
3c33dd2a2d355ee5ba0287367e209aa147a39aa00607f0c95fb2bf1ade45d014
c5b5dffe7dd8beebdc1baa8b5b05300a9f7079e65dcfd42ade6f8a77ff09537d
O=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccccc1
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[C:2](-[C:3])-[C:4](=[O;D1;H0:5])-[#8:6]-[C;D1;H3:7]>>[C:3]-[C:2](-[NH2;D1;+0:1])-[C:4](=[O;D1;H0:5])-[#8:6]-[C;D1;H3:7]
null
[]
null
null
4
HOUR
4 g of the compound obtained in Step C of Example 10 are dissolved in 200 ml of dichloromethane and the temperature is lowered to 0° C. 12.47 ml of trifluoroacetic acid are then added and the reaction mixture is stirred at ambient temperature for 4 hours. Conditions: See reaction.notes.procedure_details. Workup: is low...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Primary amine
null
null
c1ccccc1.c1ccc2scnc2c1.c1ccccc1
HO-
ClCCl
null
4
COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)OC(C)(C)C>ClCCl>COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4d27a926032c4fd3b521a094bbec068f
CCCCOC(=O)Cl.COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1>>CCCCOC(=O)NC(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)C(=O)OC
FC(C(=O)O)(F)F.NC(C(=O)OC)CC1=CC=C(C=C1)OCCN1C(SC2=C1C=CC(=C2)C(C2=CC=CC=C2)=O)=O.C(C)N(CC)CC.ClC(=O)OCCCC>>C(C1=CC=CC=C1)(=O)C1=CC2=C(N(C(S2)=O)CCOC2=CC=C(C=C2)CC(C(=O)OC)NC(=O)OCCCC)C=C1
Cl[C:6]([O:5][CH2:4][CH2:3][CH2:2][CH3:1])=[O:7].[NH2:8][CH:9]([CH2:10][c:11]1[cH:12][cH:13][c:14]([O:15][CH2:16][CH2:17][n:18]2[c:19](=[O:20])[s:21][c:22]3[cH:23][c:24]([C:25](=[O:26])[c:27]4[cH:28][cH:29][cH:30][cH:31][cH:32]4)[cH:33][cH:34][c:35]23)[cH:36][cH:37]1)[C:38](=[O:39])[O:40][CH3:41]>>[CH3:1][CH2:2][CH2:3]...
CCCCOC(=O)Cl.COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1
CCCCOC(=O)NC(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)C(=O)OC
null
null
C(C)(=O)OCC
Protection
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
038720aa61a7efa0f2a9ee6f2e0adf63a9ffdc2be4697c11a6215baef34f97b2
205f353513ce9506ab61831799da8fb73ec2ef5cfa927664496d3ce72c438860
O=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C:4].[C:5]-[C:6](-[NH2;D1;+0:7])-[C:8](=[O;D1;H0:9])-[#8:10]-[C;D1;H3:11]>>[C:5]-[C:6](-[NH;D2;+0:7]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C:4])-[C:8](=[O;D1;H0:9])-[#8:10]-[C;D1;H3:11]
null
[]
null
null
8
HOUR
700 mg of the compound obtained in Step A are dissolved in 10 ml of ethyl acetate; 0.494 ml of triethylamine is then added and the temperature is lowered to 0° C. 0.229 ml of butyl chloroformate is added and the mixture is allowed to return to ambient temperature and is stirred overnight. Conditions: See reaction.notes...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Ether.Primary amine
Carbamic ester
null
null
c1ccccc1.c1ccc2scnc2c1.c1ccccc1
HCl
C(C)(=O)OCC
null
8
CCCCOC(=O)Cl.COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1>C(C)(=O)OCC>CCCCOC(=O)NC(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)C(=O)OC
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-72dcbc5d7d0641808f1523b51fa60c26
CCCCOC(=O)NC(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)C(=O)OC.CON>>CCCCOC(=O)NC(Cc1ccc(OCCn2c(=O)sc3cc(C(=NOC)c4ccccc4)ccc32)cc1)C(=O)OC
C(C1=CC=CC=C1)(=O)C1=CC2=C(N(C(S2)=O)CCOC2=CC=C(C=C2)CC(C(=O)OC)NC(=O)OCCCC)C=C1.CON>>C(CCC)OC(=O)NC(C(=O)OC)CC1=CC=C(C=C1)OCCN1C(SC2=C1C=CC(=C2)C(C2=CC=CC=C2)=NOC)=O
O=[C:25]([c:24]1[cH:23][c:22]2[s:21][c:19](=[O:20])[n:18]([CH2:17][CH2:16][O:15][c:14]3[cH:13][cH:12][c:11]([CH2:10][CH:9]([NH:8][C:6]([O:5][CH2:4][CH2:3][CH2:2][CH3:1])=[O:7])[C:40](=[O:41])[O:42][CH3:43])[cH:39][cH:38]3)[c:37]2[cH:36][cH:35]1)[c:29]1[cH:30][cH:31][cH:32][cH:33][cH:34]1.[NH2:26][O:27][CH3:28]>>[CH3:1]...
CCCCOC(=O)NC(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)C(=O)OC.CON
CCCCOC(=O)NC(Cc1ccc(OCCn2c(=O)sc3cc(C(=NOC)c4ccccc4)ccc32)cc1)C(=O)OC
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
3d7a74a3d1c5abb5292963d4a3067f1fb8a89aead752dc9bb1d63522c4c0bd5c
6b0edeaa66853687109d0d530554f76edf36b01a8ec084e7ae9c709f0949a6b9
N=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccccc1
O=[C;H0;D3;+0:1](-[c:2](:[c:3]):[c:4]:[c:5]:[#16;a:6])-[c:7](:[c:8]):[c:9].[C;D1;H3:10]-[#8:11]-[NH2;D1;+0:12]>>[#16;a:6]:[c:5]:[c:4]:[c:2](-[C;H0;D3;+0:1](=[N;H0;D2;+0:12]-[#8:11]-[C;D1;H3:10])-[c:7](:[c:8]):[c:9]):[c:3]
null
[]
null
null
null
null
Starting from the compound obtained in Step B, the procedure is as in Step B of Example 2, replacing the hydroxylamine by O-methylhydroxylamine. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Ketone.Primary amine
null
null
null
c1ccccc1.c1ccc2scnc2c1.c1ccccc1
HO-
null
null
null
CCCCOC(=O)NC(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)C(=O)OC.CON>>CCCCOC(=O)NC(Cc1ccc(OCCn2c(=O)sc3cc(C(=NOC)c4ccccc4)ccc32)cc1)C(=O)OC
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-13992fe0befe48999b1f2b27de427aba
COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1.O=C(Cl)Oc1ccccc1>>COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)Oc1ccccc1
FC(C(=O)O)(F)F.NC(C(=O)OC)CC1=CC=C(C=C1)OCCN1C(SC2=C1C=CC(=C2)C(C2=CC=CC=C2)=O)=O.C(C)N(CC)CC.ClC(=O)OC1=CC=CC=C1>>C(C1=CC=CC=C1)(=O)C1=CC2=C(N(C(S2)=O)CCOC2=CC=C(C=C2)CC(C(=O)OC)NC(=O)OC2=CC=CC=C2)C=C1
[CH3:1][O:2][C:3](=[O:4])[CH:5]([CH2:6][c:7]1[cH:8][cH:9][c:10]([O:11][CH2:12][CH2:13][n:14]2[c:15](=[O:16])[s:17][c:18]3[cH:19][c:20]([C:21](=[O:22])[c:23]4[cH:24][cH:25][cH:26][cH:27][cH:28]4)[cH:29][cH:30][c:31]23)[cH:32][cH:33]1)[NH2:34].Cl[C:35](=[O:36])[O:37][c:38]1[cH:39][cH:40][cH:41][cH:42][cH:43]1>>[CH3:1][O:...
COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1.O=C(Cl)Oc1ccccc1
COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)Oc1ccccc1
null
null
C(C)(=O)OCC
Protection
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
038720aa61a7efa0f2a9ee6f2e0adf63a9ffdc2be4697c11a6215baef34f97b2
205f353513ce9506ab61831799da8fb73ec2ef5cfa927664496d3ce72c438860
O=C(NCCc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)Oc1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[c:4].[C:5]-[C:6](-[NH2;D1;+0:7])-[C:8](=[O;D1;H0:9])-[#8:10]-[C;D1;H3:11]>>[C:5]-[C:6](-[NH;D2;+0:7]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[c:4])-[C:8](=[O;D1;H0:9])-[#8:10]-[C;D1;H3:11]
null
[]
null
null
8
HOUR
1.5 g of the compound obtained in Step A of Example 12 are dissolved in 20 ml of ethyl acetate; 1.06 ml of triethylamine are then added and the temperature is lowered to 0° C. 0.637 ml of phenyl chloroformate is then added and the mixture is allowed to return to ambient temperature and is stirred overnight. Conditions:...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Ether.Primary amine
Carbamic ester
null
null
c1ccccc1.c1ccc2scnc2c1.c1ccccc1.c1ccccc1
HCl
C(C)(=O)OCC
null
8
COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1.O=C(Cl)Oc1ccccc1>C(C)(=O)OCC>COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)Oc1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c72ed27bd59f40559ae816b565ea20b1
COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)Oc1ccccc1.CON>>CON=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccc(CC(NC(=O)Oc2ccccc2)C(=O)OC)cc1
C(C1=CC=CC=C1)(=O)C1=CC2=C(N(C(S2)=O)CCOC2=CC=C(C=C2)CC(C(=O)OC)NC(=O)OC2=CC=CC=C2)C=C1.CON>>CON=C(C1=CC2=C(N(C(S2)=O)CCOC2=CC=C(C=C2)CC(C(=O)OC)NC(=O)OC2=CC=CC=C2)C=C1)C1=CC=CC=C1
O=[C:4]([c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1)[c:11]1[cH:12][cH:13][c:14]2[c:15]([cH:16]1)[s:17][c:18](=[O:19])[n:20]2[CH2:21][CH2:22][O:23][c:24]1[cH:25][cH:26][c:27]([CH2:28][CH:29]([NH:30][C:31](=[O:32])[O:33][c:34]2[cH:35][cH:36][cH:37][cH:38][cH:39]2)[C:40](=[O:41])[O:42][CH3:43])[cH:44][cH:45]1.[CH3:1][O:2][NH2:...
COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)Oc1ccccc1.CON
CON=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccc(CC(NC(=O)Oc2ccccc2)C(=O)OC)cc1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
3d7a74a3d1c5abb5292963d4a3067f1fb8a89aead752dc9bb1d63522c4c0bd5c
6b0edeaa66853687109d0d530554f76edf36b01a8ec084e7ae9c709f0949a6b9
N=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccc(CCNC(=O)Oc2ccccc2)cc1
O=[C;H0;D3;+0:1](-[c:2](:[c:3]):[c:4]:[c:5]:[#16;a:6])-[c:7](:[c:8]):[c:9].[C;D1;H3:10]-[#8:11]-[NH2;D1;+0:12]>>[#16;a:6]:[c:5]:[c:4]:[c:2](-[C;H0;D3;+0:1](=[N;H0;D2;+0:12]-[#8:11]-[C;D1;H3:10])-[c:7](:[c:8]):[c:9]):[c:3]
null
[]
null
null
null
null
Starting from the compound obtained in Step A, the procedure is as in Step B of Example 2, replacing the hydroxylamine by O-methylhydroxylamine. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Ketone.Primary amine
null
null
null
c1ccccc1.c1ccc2scnc2c1.c1ccccc1.c1ccccc1
HO-
null
null
null
COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)Oc1ccccc1.CON>>CON=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccc(CC(NC(=O)Oc2ccccc2)C(=O)OC)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-36a2284b3914451da4caa41aaa3484ca
COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1.O=C(Cl)OCc1ccccc1>>COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)OCc1ccccc1
FC(C(=O)O)(F)F.NC(C(=O)OC)CC1=CC=C(C=C1)OCCN1C(SC2=C1C=CC(=C2)C(C2=CC=CC=C2)=O)=O.C(C)N(CC)CC.ClC(=O)OCC1=CC=CC=C1>>C(C1=CC=CC=C1)(=O)C1=CC2=C(N(C(S2)=O)CCOC2=CC=C(C=C2)CC(C(=O)OC)NC(=O)OCC2=CC=CC=C2)C=C1
[CH3:1][O:2][C:3](=[O:4])[CH:5]([CH2:6][c:7]1[cH:8][cH:9][c:10]([O:11][CH2:12][CH2:13][n:14]2[c:15](=[O:16])[s:17][c:18]3[cH:19][c:20]([C:21](=[O:22])[c:23]4[cH:24][cH:25][cH:26][cH:27][cH:28]4)[cH:29][cH:30][c:31]23)[cH:32][cH:33]1)[NH2:34].Cl[C:35](=[O:36])[O:37][CH2:38][c:39]1[cH:40][cH:41][cH:42][cH:43][cH:44]1>>[C...
COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1.O=C(Cl)OCc1ccccc1
COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)OCc1ccccc1
null
null
C(C)(=O)OCC
Protection
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
038720aa61a7efa0f2a9ee6f2e0adf63a9ffdc2be4697c11a6215baef34f97b2
205f353513ce9506ab61831799da8fb73ec2ef5cfa927664496d3ce72c438860
O=C(NCCc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)OCc1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C:4].[C:5]-[C:6](-[NH2;D1;+0:7])-[C:8](=[O;D1;H0:9])-[#8:10]-[C;D1;H3:11]>>[C:4]-[#8:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:7]-[C:6](-[C:5])-[C:8](=[O;D1;H0:9])-[#8:10]-[C;D1;H3:11]
null
[]
null
null
8
HOUR
1.5 g of the compound obtained in Step A of Example 12 are dissolved in 20 ml of ethyl acetate; 1.06 ml of triethylamine are then added and the temperature is lowered to 0° C. 0.725 ml of benzyl chloroformate are added and the mixture is allowed to return to ambient temperature and is stirred overnight. Conditions: See...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Ether.Primary amine
Carbamic ester
null
null
c1ccccc1.c1ccc2scnc2c1.c1ccccc1.c1ccccc1
HCl
C(C)(=O)OCC
null
8
COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1.O=C(Cl)OCc1ccccc1>C(C)(=O)OCC>COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)OCc1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d82f864ac1fb47c593bfbc678401124d
CC(=O)Cl.COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1>>COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(C)=O
FC(C(=O)O)(F)F.NC(C(=O)OC)CC1=CC=C(C=C1)OCCN1C(SC2=C1C=CC(=C2)C(C2=CC=CC=C2)=O)=O.C(C)N(CC)CC.C(C)(=O)Cl>>C(C)(=O)NC(C(=O)OC)CC1=CC=C(C=C1)OCCN1C(SC2=C1C=CC(=C2)C(C2=CC=CC=C2)=O)=O
Cl[C:35]([CH3:36])=[O:37].[CH3:1][O:2][C:3](=[O:4])[CH:5]([CH2:6][c:7]1[cH:8][cH:9][c:10]([O:11][CH2:12][CH2:13][n:14]2[c:15](=[O:16])[s:17][c:18]3[cH:19][c:20]([C:21](=[O:22])[c:23]4[cH:24][cH:25][cH:26][cH:27][cH:28]4)[cH:29][cH:30][c:31]23)[cH:32][cH:33]1)[NH2:34]>>[CH3:1][O:2][C:3](=[O:4])[CH:5]([CH2:6][c:7]1[cH:8]...
CC(=O)Cl.COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1
COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(C)=O
null
null
C(C)(=O)OCC
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
O=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccccc1
Cl-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[C:4]-[C:5](-[NH2;D1;+0:6])-[C:7](=[O;D1;H0:8])-[#8:9]-[C;D1;H3:10]>>[C:4]-[C:5](-[NH;D2;+0:6]-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3])-[C:7](=[O;D1;H0:8])-[#8:9]-[C;D1;H3:10]
null
[]
null
null
8
HOUR
500 mg of the compound obtained in Step A of Example 12 are dissolved in 10 ml of ethyl acetate; 0.353 ml of triethylamine is then added and the temperature is lowered to 0° C. 0.121 ml of acetyl chloride is added and the mixture is allowed to return to ambient temperature and is stirred overnight. Conditions: See reac...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccc2scnc2c1.c1ccccc1
HCl
C(C)(=O)OCC
null
8
CC(=O)Cl.COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1>C(C)(=O)OCC>COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(C)=O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-fc6f7c8c4ba2404bbed671328fca3321
COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(C)=O.CON>>CON=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccc(CC(NC(C)=O)C(=O)OC)cc1
C(C)(=O)NC(C(=O)OC)CC1=CC=C(C=C1)OCCN1C(SC2=C1C=CC(=C2)C(C2=CC=CC=C2)=O)=O.CON>>C(C)(=O)NC(C(=O)OC)CC1=CC=C(C=C1)OCCN1C(SC2=C1C=CC(=C2)C(C2=CC=CC=C2)=NOC)=O
O=[C:4]([c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1)[c:11]1[cH:12][cH:13][c:14]2[c:15]([cH:16]1)[s:17][c:18](=[O:19])[n:20]2[CH2:21][CH2:22][O:23][c:24]1[cH:25][cH:26][c:27]([CH2:28][CH:29]([NH:30][C:31]([CH3:32])=[O:33])[C:34](=[O:35])[O:36][CH3:37])[cH:38][cH:39]1.[CH3:1][O:2][NH2:3]>>[CH3:1][O:2][N:3]=[C:4]([c:5]1[cH:6][...
COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(C)=O.CON
CON=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccc(CC(NC(C)=O)C(=O)OC)cc1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
3d7a74a3d1c5abb5292963d4a3067f1fb8a89aead752dc9bb1d63522c4c0bd5c
6b0edeaa66853687109d0d530554f76edf36b01a8ec084e7ae9c709f0949a6b9
N=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccccc1
O=[C;H0;D3;+0:1](-[c:2](:[c:3]):[c:4]:[c:5]:[#16;a:6])-[c:7](:[c:8]):[c:9].[C;D1;H3:10]-[#8:11]-[NH2;D1;+0:12]>>[#16;a:6]:[c:5]:[c:4]:[c:2](-[C;H0;D3;+0:1](=[N;H0;D2;+0:12]-[#8:11]-[C;D1;H3:10])-[c:7](:[c:8]):[c:9]):[c:3]
null
[]
null
null
null
null
Starting from the compound obtained in Step A, the procedure is as in Step B of Example 2, replacing the hydroxylamine by O-methylhydroxylamine. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Ketone.Primary amine
null
null
null
c1ccccc1.c1ccc2scnc2c1.c1ccccc1
HO-
null
null
null
COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(C)=O.CON>>CON=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccc(CC(NC(C)=O)C(=O)OC)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5d99a487dd824cc1886a6c201ec4a455
CCCC(=O)Cl.COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1>>CCCC(=O)NC(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)C(=O)OC
FC(C(=O)O)(F)F.NC(C(=O)OC)CC1=CC=C(C=C1)OCCN1C(SC2=C1C=CC(=C2)C(C2=CC=CC=C2)=O)=O.C(C)N(CC)CC.C(CCC)(=O)Cl>>C(C1=CC=CC=C1)(=O)C1=CC2=C(N(C(S2)=O)CCOC2=CC=C(C=C2)CC(C(=O)OC)NC(CCC)=O)C=C1
Cl[C:4]([CH2:3][CH2:2][CH3:1])=[O:5].[NH2:6][CH:7]([CH2:8][c:9]1[cH:10][cH:11][c:12]([O:13][CH2:14][CH2:15][n:16]2[c:17](=[O:18])[s:19][c:20]3[cH:21][c:22]([C:23](=[O:24])[c:25]4[cH:26][cH:27][cH:28][cH:29][cH:30]4)[cH:31][cH:32][c:33]23)[cH:34][cH:35]1)[C:36](=[O:37])[O:38][CH3:39]>>[CH3:1][CH2:2][CH2:3][C:4](=[O:5])[...
CCCC(=O)Cl.COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1
CCCC(=O)NC(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)C(=O)OC
null
null
C(C)(=O)OCC
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
O=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4].[C:5]-[C:6](-[NH2;D1;+0:7])-[C:8](=[O;D1;H0:9])-[#8:10]-[C;D1;H3:11]>>[C:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:7]-[C:6](-[C:5])-[C:8](=[O;D1;H0:9])-[#8:10]-[C;D1;H3:11]
null
[]
null
null
8
HOUR
500 mg of the compound obtained in Step A of Example 12 are dissolved in 10 ml of ethyl acetate; 0.353 ml of triethylamine is then added and the temperature is lowered to 0° C. 0.177 ml of butyryl chloride is added and the mixture is allowed to return to ambient temperature and is stirred overnight. Conditions: See rea...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccc2scnc2c1.c1ccccc1
HCl
C(C)(=O)OCC
null
8
CCCC(=O)Cl.COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1>C(C)(=O)OCC>CCCC(=O)NC(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)C(=O)OC
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b8c38dab124e4d2190af98e5b41f45d6
COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1.O=C(Cl)c1ccccc1>>COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)c1ccccc1
FC(C(=O)O)(F)F.NC(C(=O)OC)CC1=CC=C(C=C1)OCCN1C(SC2=C1C=CC(=C2)C(C2=CC=CC=C2)=O)=O.C(C)N(CC)CC.C(C1=CC=CC=C1)(=O)Cl>>C(C1=CC=CC=C1)(=O)NC(C(=O)OC)CC1=CC=C(C=C1)OCCN1C(SC2=C1C=CC(=C2)C(C2=CC=CC=C2)=O)=O
[CH3:1][O:2][C:3](=[O:4])[CH:5]([CH2:6][c:7]1[cH:8][cH:9][c:10]([O:11][CH2:12][CH2:13][n:14]2[c:15](=[O:16])[s:17][c:18]3[cH:19][c:20]([C:21](=[O:22])[c:23]4[cH:24][cH:25][cH:26][cH:27][cH:28]4)[cH:29][cH:30][c:31]23)[cH:32][cH:33]1)[NH2:34].Cl[C:35](=[O:36])[c:37]1[cH:38][cH:39][cH:40][cH:41][cH:42]1>>[CH3:1][O:2][C:3...
COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1.O=C(Cl)c1ccccc1
COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)c1ccccc1
null
null
C(C)(=O)OCC
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
O=C(NCCc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)c1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C:6]-[C:7](-[NH2;D1;+0:8])-[C:9](=[O;D1;H0:10])-[#8:11]-[C;D1;H3:12]>>[C:6]-[C:7](-[NH;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5])-[C:9](=[O;D1;H0:10])-[#8:11]-[C;D1;H3:12]
null
[]
null
null
8
HOUR
500 mg of the compound obtained in Step A of Example 12 are dissolved in 10 ml of ethyl acetate; 0.353 ml of triethylamine is then added and the temperature is lowered to 0° C. 0.197 ml of benzoyl chloride is added and the mixture is allowed to return to ambient temperature and is stirred overnight. Conditions: See rea...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccc2scnc2c1.c1ccccc1.c1ccccc1
HCl
C(C)(=O)OCC
null
8
COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1.O=C(Cl)c1ccccc1>C(C)(=O)OCC>COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)c1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ffab1b33acd54a0e919e87ad681cd354
COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1.O=C(Cl)Cc1ccccc1>>COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)Cc1ccccc1
FC(C(=O)O)(F)F.NC(C(=O)OC)CC1=CC=C(C=C1)OCCN1C(SC2=C1C=CC(=C2)C(C2=CC=CC=C2)=O)=O.C(C)N(CC)CC.C1(=CC=CC=C1)CC(=O)Cl>>C(C1=CC=CC=C1)(=O)C1=CC2=C(N(C(S2)=O)CCOC2=CC=C(C=C2)CC(C(=O)OC)NC(CC2=CC=CC=C2)=O)C=C1
[CH3:1][O:2][C:3](=[O:4])[CH:5]([CH2:6][c:7]1[cH:8][cH:9][c:10]([O:11][CH2:12][CH2:13][n:14]2[c:15](=[O:16])[s:17][c:18]3[cH:19][c:20]([C:21](=[O:22])[c:23]4[cH:24][cH:25][cH:26][cH:27][cH:28]4)[cH:29][cH:30][c:31]23)[cH:32][cH:33]1)[NH2:34].Cl[C:35](=[O:36])[CH2:37][c:38]1[cH:39][cH:40][cH:41][cH:42][cH:43]1>>[CH3:1][...
COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1.O=C(Cl)Cc1ccccc1
COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)Cc1ccccc1
null
null
C(C)(=O)OCC
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
O=C(Cc1ccccc1)NCCc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[c:4].[C:5]-[C:6](-[NH2;D1;+0:7])-[C:8](=[O;D1;H0:9])-[#8:10]-[C;D1;H3:11]>>[C:5]-[C:6](-[NH;D2;+0:7]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[c:4])-[C:8](=[O;D1;H0:9])-[#8:10]-[C;D1;H3:11]
null
[]
null
null
8
HOUR
500 mg of the compound obtained in Step A of Example 12 are dissolved in 10 ml of ethyl acetate; 0.353 ml of triethylamine is then added and the temperature is lowered to 0° C. 0.226 ml of phenylacetyl chloride is added and the mixture is allowed to return to ambient temperature and is stirred overnight. Conditions: Se...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccc2scnc2c1.c1ccccc1.c1ccccc1
HCl
C(C)(=O)OCC
null
8
COC(=O)C(N)Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1.O=C(Cl)Cc1ccccc1>C(C)(=O)OCC>COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)Cc1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5bb22604b46646c795135d0fe0712371
COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)Cc1ccccc1.CON>>CON=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccc(CC(NC(=O)Cc2ccccc2)C(=O)OC)cc1
C(C1=CC=CC=C1)(=O)C1=CC2=C(N(C(S2)=O)CCOC2=CC=C(C=C2)CC(C(=O)OC)NC(CC2=CC=CC=C2)=O)C=C1.CON>>CON=C(C1=CC2=C(N(C(S2)=O)CCOC2=CC=C(C=C2)CC(C(=O)OC)NC(CC2=CC=CC=C2)=O)C=C1)C1=CC=CC=C1
O=[C:4]([c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1)[c:11]1[cH:12][cH:13][c:14]2[c:15]([cH:16]1)[s:17][c:18](=[O:19])[n:20]2[CH2:21][CH2:22][O:23][c:24]1[cH:25][cH:26][c:27]([CH2:28][CH:29]([NH:30][C:31](=[O:32])[CH2:33][c:34]2[cH:35][cH:36][cH:37][cH:38][cH:39]2)[C:40](=[O:41])[O:42][CH3:43])[cH:44][cH:45]1.[CH3:1][O:2][NH...
COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)Cc1ccccc1.CON
CON=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccc(CC(NC(=O)Cc2ccccc2)C(=O)OC)cc1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
3d7a74a3d1c5abb5292963d4a3067f1fb8a89aead752dc9bb1d63522c4c0bd5c
6b0edeaa66853687109d0d530554f76edf36b01a8ec084e7ae9c709f0949a6b9
N=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccc(CCNC(=O)Cc2ccccc2)cc1
O=[C;H0;D3;+0:1](-[c:2](:[c:3]):[c:4]:[c:5]:[#16;a:6])-[c:7](:[c:8]):[c:9].[C;D1;H3:10]-[#8:11]-[NH2;D1;+0:12]>>[#16;a:6]:[c:5]:[c:4]:[c:2](-[C;H0;D3;+0:1](=[N;H0;D2;+0:12]-[#8:11]-[C;D1;H3:10])-[c:7](:[c:8]):[c:9]):[c:3]
null
[]
null
null
null
null
Starting from the compound obtained in Step A, the procedure is as in Step B of Example 2, replacing the hydroxylamine by O-methylhydroxylamine. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Ketone.Primary amine
null
null
null
c1ccccc1.c1ccc2scnc2c1.c1ccccc1.c1ccccc1
HO-
null
null
null
COC(=O)C(Cc1ccc(OCCn2c(=O)sc3cc(C(=O)c4ccccc4)ccc32)cc1)NC(=O)Cc1ccccc1.CON>>CON=C(c1ccccc1)c1ccc2c(c1)sc(=O)n2CCOc1ccc(CC(NC(=O)Cc2ccccc2)C(=O)OC)cc1