dataset_id
large_stringclasses
414 values
reaction_id
large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
reactant_smiles
large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-8c5fd294e6cf401c9bc897f31628a4c5
C[C@@H]1CC[C@@H](NC(=O)OC(C)(C)C)[C@H](O)CN1S(=O)(=O)c1ccccn1>>C[C@@H]1CC[C@@H](N)[C@H](O)CN1S(=O)(=O)c1ccccn1
Cl.C(C)(C)(C)OC(N[C@H]1[C@@H](CN([C@@H](CC1)C)S(=O)(=O)C1=NC=CC=C1)O)=O>>N[C@H]1[C@@H](CN([C@@H](CC1)C)S(=O)(=O)C1=NC=CC=C1)O
CC(C)(C)OC(=O)[NH:6][C@@H:5]1[CH2:4][CH2:3][C@@H:2]([CH3:1])[N:10]([S:11](=[O:12])(=[O:13])[c:14]2[cH:15][cH:16][cH:17][cH:18][n:19]2)[CH2:9][C@H:7]1[OH:8]>>[CH3:1][C@@H:2]1[CH2:3][CH2:4][C@@H:5]([NH2:6])[C@H:7]([OH:8])[CH2:9][N:10]1[S:11](=[O:12])(=[O:13])[c:14]1[cH:15][cH:16][cH:17][cH:18][n:19]1
C[C@@H]1CC[C@@H](NC(=O)OC(C)(C)C)[C@H](O)CN1S(=O)(=O)c1ccccn1
C[C@@H]1CC[C@@H](N)[C@H](O)CN1S(=O)(=O)c1ccccn1
null
null
O1CCOCC1.C1(=CC=CC=C1)C.CO
Reduction
Hydrogenolysis of amides/imides/carbamates
3c33dd2a2d355ee5ba0287367e209aa147a39aa00607f0c95fb2bf1ade45d014
c5b5dffe7dd8beebdc1baa8b5b05300a9f7079e65dcfd42ade6f8a77ff09537d
O=S(=O)(c1ccccn1)N1CCCCCC1
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[C:2](-[C:3])-[C:4]>>[C:3]-[C:2](-[NH2;D1;+0:1])-[C:4]
null
[]
null
null
1
HOUR
HCl in dioxane (4.0 M, 10 ml) was added to a stirred solution. [(3R,4R,7R)-3-Hydroxy-7-methyl-1-(pyridine-2-sulfonyl)-azepan-4-yl]-carbamic acid tert-butyl ester (0.6 g, 1.55 mmol) in MeOH (10 ml). The reaction mixture was stirred for 1 h at RT, then was diluted with toluene (20 ml), concentrated in vacuo by rotary eva...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Primary amine
null
null
C1CCC[NH]CC1.c1ccncc1
HO-
O1CCOCC1.C1(=CC=CC=C1)C.CO
null
1
C[C@@H]1CC[C@@H](NC(=O)OC(C)(C)C)[C@H](O)CN1S(=O)(=O)c1ccccn1>O1CCOCC1.C1(=CC=CC=C1)C.CO>C[C@@H]1CC[C@@H](N)[C@H](O)CN1S(=O)(=O)c1ccccn1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-88e1ce2fbff54f2cb450c53d5c5fc09d
CC(C)CC(C(=O)O)c1cccc(-c2ccccc2)c1.C[C@@H]1CC[C@@H](N)[C@H](O)CN1S(=O)(=O)c1ccccn1>>CC(C)CC(C(=O)N[C@@H]1CC[C@@H](C)N(S(=O)(=O)c2ccccn2)C[C@H]1O)c1cccc(-c2ccccc2)c1
C1(=CC(=CC=C1)C(C(=O)O)CC(C)C)C1=CC=CC=C1.N[C@H]1[C@@H](CN([C@@H](CC1)C)S(=O)(=O)C1=NC=CC=C1)O.CCN=C=NCCCN(C)C.C=1C=CC2=C(C1)N=NN2O.C(C)(C)N(CC)C(C)C>>C[C@@H]1CC[C@H]([C@@H](CN1S(=O)(=O)C1=NC=CC=C1)O)NC(C(CC(C)C)C=1C=C(C=CC1)C1=CC=CC=C1)=O
O[C:6]([CH:5]([CH2:4][CH:2]([CH3:1])[CH3:3])[c:27]1[cH:28][cH:29][cH:30][c:31](-[c:32]2[cH:33][cH:34][cH:35][cH:36][cH:37]2)[cH:38]1)=[O:7].[NH2:8][C@@H:9]1[CH2:10][CH2:11][C@@H:12]([CH3:13])[N:14]([S:15](=[O:16])(=[O:17])[c:18]2[cH:19][cH:20][cH:21][cH:22][n:23]2)[CH2:24][C@H:25]1[OH:26]>>[CH3:1][CH:2]([CH3:3])[CH2:4]...
CC(C)CC(C(=O)O)c1cccc(-c2ccccc2)c1.C[C@@H]1CC[C@@H](N)[C@H](O)CN1S(=O)(=O)c1ccccn1
CC(C)CC(C(=O)N[C@@H]1CC[C@@H](C)N(S(=O)(=O)c2ccccn2)C[C@H]1O)c1cccc(-c2ccccc2)c1
null
null
CN(C)C=O.CCOC(=O)C
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(Cc1cccc(-c2ccccc2)c1)N[C@@H]1CCCN(S(=O)(=O)c2ccccn2)CC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[c:5].[C:6]-[C:7](-[NH2;D1;+0:8])-[C:9]>>[C:6]-[C:7](-[NH;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[c:5])-[C:9]
62
[{"value": 62.0, "product": "C[C@@H]1CC[C@H]([C@@H](CN1S(=O)(=O)C1=NC=CC=C1)O)NC(C(CC(C)C)C=1C=C(C=CC1)C1=CC=CC=C1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 61.6, "product": "C[C@@H]1CC[C@H]([C@@H](CN1S(=O)(=O)C1=NC=CC=C1)O)NC(C(CC(C)C)C=1C=C(C=CC1)C1=CC=CC=C1)=O", "details": "CALCULATEDPERCENTYIE...
null
null
null
null
2-Biphenyl-3-yl-4-methyl-pentanoic acid (270 mg, 1.0 mmol, preparation described in J. Am. Chem. Soc. 1997, 120, 9114), and (3R,4R,7R)-4-Amino-7-methyl-1-(pyridine-2-sulfonyl)-azepan-3-ol (320 mg, 1.0mmol, Example 1k), EDCI (190 mg, 1.0 mmol), HOBT (135 mg, 1.0 mmol) and diisopropylethylamine (1.7 g, 0.23 ml, 1.3 mmol)...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
C1CCC[NH]CC1.c1ccncc1.c1ccccc1.c1ccccc1
HO-
CN(C)C=O.CCOC(=O)C
null
null
CC(C)CC(C(=O)O)c1cccc(-c2ccccc2)c1.C[C@@H]1CC[C@@H](N)[C@H](O)CN1S(=O)(=O)c1ccccn1>CN(C)C=O.CCOC(=O)C>CC(C)CC(C(=O)N[C@@H]1CC[C@@H](C)N(S(=O)(=O)c2ccccn2)C[C@H]1O)c1cccc(-c2ccccc2)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-963533c2871343e58992cbadacb6eca0
CNC(=O)c1cc(Cl)ccn1.Nc1ccc(O)cc1[N+](=O)[O-]>>CNC(=O)c1cc(Oc2ccc(N)c([N+](=O)[O-])c2)ccn1
NC1=C(C=C(C=C1)O)[N+](=O)[O-].C[Si](C)(C)[N-][Si](C)(C)C.[K+].ClC1=CC(=NC=C1)C(=O)NC.C([O-])([O-])=O.[K+].[K+]>>NC1=C(C=C(C=C1)OC1=CC(=NC=C1)C(=O)NC)[N+](=O)[O-]
Cl[c:7]1[cH:6][c:5]([C:3]([NH:2][CH3:1])=[O:4])[n:21][cH:20][cH:19]1.[OH:8][c:9]1[cH:10][cH:11][c:12]([NH2:13])[c:14]([N+:15](=[O:16])[O-:17])[cH:18]1>>[CH3:1][NH:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([O:8][c:9]2[cH:10][cH:11][c:12]([NH2:13])[c:14]([N+:15](=[O:16])[O-:17])[cH:18]2)[cH:19][cH:20][n:21]1
CNC(=O)c1cc(Cl)ccn1.Nc1ccc(O)cc1[N+](=O)[O-]
CNC(=O)c1cc(Oc2ccc(N)c([N+](=O)[O-])c2)ccn1
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
99925b30dd2603ae575cba81b58435d015cd6b7267cf347380904f25833af5f2
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1ccc(Oc2ccncc2)cc1
Cl-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[#7;a:4]:[c:5](-[C:6](-[#7:7])=[O;D1;H0:8]):[c:9]:1.[OH;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[#7:7]-[C:6](=[O;D1;H0:8])-[c:5]1:[#7;a:4]:[c:3]:[c:2]:[c;H0;D3;+0:1](-[O;H0;D2;+0:10]-[c:11](:[c:12]):[c:13]):[c:9]:1
null
[]
90
CELSIUS
3
DAY
A mixture containing 4-amino-3-nitrophenol (1 eq) and potassium bis(trimethylsilyl)amide (2 eq) was stirred in dimethylformamide for 2 hours at room temperature. To this mixture was added (4-chloro(2-pyridyl))-N-methylcarboxamide (1 eq) and potassium carbonate (1.2 eq) and stirred at 90° C. for 3 days. The reaction mix...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccncc1
c1ccncc1
c1ccncc1.c1ccccc1
HCl
CN(C=O)C
90
72
CNC(=O)c1cc(Cl)ccn1.Nc1ccc(O)cc1[N+](=O)[O-]>CN(C=O)C>CNC(=O)c1cc(Oc2ccc(N)c([N+](=O)[O-])c2)ccn1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-da96264e0f81436bab3b63be0e66a636
CNC(=O)c1cc(Cl)ccn1.Oc1ccc2sc(Nc3ccc(Br)cc3)nc2c1>>CNC(=O)c1cc(Oc2ccc3sc(Nc4ccc(Br)cc4)nc3c2)ccn1
BrC1=CC=C(C=C1)NC=1SC2=C(N1)C=C(C=C2)O.C[Si](C)(C)[N-][Si](C)(C)C.[K+].ClC1=CC(=NC=C1)C(=O)NC.C([O-])([O-])=O.[K+].[K+]>>BrC1=CC=C(C=C1)NC=1SC2=C(N1)C=C(C=C2)OC2=CC(=NC=C2)C(=O)NC
Cl[c:7]1[cH:6][c:5]([C:3]([NH:2][CH3:1])=[O:4])[n:28][cH:27][cH:26]1.[OH:8][c:9]1[cH:10][cH:11][c:12]2[s:13][c:14]([NH:15][c:16]3[cH:17][cH:18][c:19]([Br:20])[cH:21][cH:22]3)[n:23][c:24]2[cH:25]1>>[CH3:1][NH:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([O:8][c:9]2[cH:10][cH:11][c:12]3[s:13][c:14]([NH:15][c:16]4[cH:17][cH:18][c:19]...
CNC(=O)c1cc(Cl)ccn1.Oc1ccc2sc(Nc3ccc(Br)cc3)nc2c1
CNC(=O)c1cc(Oc2ccc3sc(Nc4ccc(Br)cc4)nc3c2)ccn1
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
99925b30dd2603ae575cba81b58435d015cd6b7267cf347380904f25833af5f2
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1ccc(Nc2nc3cc(Oc4ccncc4)ccc3s2)cc1
Cl-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[#7;a:4]:[c:5](-[C:6](-[#7:7])=[O;D1;H0:8]):[c:9]:1.[#7;a:10]:[c:11]:[c:12]:[c:13](-[OH;D1;+0:14]):[c:15]>>[#7:7]-[C:6](=[O;D1;H0:8])-[c:5]1:[#7;a:4]:[c:3]:[c:2]:[c;H0;D3;+0:1](-[O;H0;D2;+0:14]-[c:13](:[c:15]):[c:12]:[c:11]:[#7;a:10]):[c:9]:1
null
[]
null
null
null
null
The mixture containing 2-[(4-bromophenyl)amino]benzothiazol-5-ol (1 eq), Potassiumbis(trimethylsilyl)amide (4 eq), was stirred in dimethylformamide for 30 min at room temperature. To this mixture was added (4-chloro(2-pyridyl)-N-methyl-carboxamide (1 eq) and Potassium carbonate (1.2 eq) and microwaved for 6 mins at 150...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccncc1
c1ccncc1
c1ccncc1.c1ccc2scnc2c1.c1ccccc1
HCl
CN(C=O)C
null
null
CNC(=O)c1cc(Cl)ccn1.Oc1ccc2sc(Nc3ccc(Br)cc3)nc2c1>CN(C=O)C>CNC(=O)c1cc(Oc2ccc3sc(Nc4ccc(Br)cc4)nc3c2)ccn1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-071bdbcaee6d468c9d5c289c3f9d91f7
CNC(=O)c1cc(Cl)ccn1.Nc1ccc(O)cc1[N+](=O)[O-]>>CNC(=O)c1cc(Oc2ccc(N)c([N+](=O)[O-])c2)ccn1
NC1=C(C=C(C=C1)O)[N+](=O)[O-].C[Si](C)(C)[N-][Si](C)(C)C.[K+].ClC1=CC(=NC=C1)C(=O)NC.C([O-])([O-])=O.[K+].[K+]>>NC1=C(C=C(OC2=CC(=NC=C2)C(=O)NC)C=C1)[N+](=O)[O-]
Cl[c:7]1[cH:6][c:5]([C:3]([NH:2][CH3:1])=[O:4])[n:21][cH:20][cH:19]1.[OH:8][c:9]1[cH:10][cH:11][c:12]([NH2:13])[c:14]([N+:15](=[O:16])[O-:17])[cH:18]1>>[CH3:1][NH:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([O:8][c:9]2[cH:10][cH:11][c:12]([NH2:13])[c:14]([N+:15](=[O:16])[O-:17])[cH:18]2)[cH:19][cH:20][n:21]1
CNC(=O)c1cc(Cl)ccn1.Nc1ccc(O)cc1[N+](=O)[O-]
CNC(=O)c1cc(Oc2ccc(N)c([N+](=O)[O-])c2)ccn1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
99925b30dd2603ae575cba81b58435d015cd6b7267cf347380904f25833af5f2
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1ccc(Oc2ccncc2)cc1
Cl-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[#7;a:4]:[c:5](-[C:6](-[#7:7])=[O;D1;H0:8]):[c:9]:1.[OH;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[#7:7]-[C:6](=[O;D1;H0:8])-[c:5]1:[#7;a:4]:[c:3]:[c:2]:[c;H0;D3;+0:1](-[O;H0;D2;+0:10]-[c:11](:[c:12]):[c:13]):[c:9]:1
72
[{"value": 72.0, "product": "NC1=C(C=C(OC2=CC(=NC=C2)C(=O)NC)C=C1)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 70.5, "product": "NC1=C(C=C(OC2=CC(=NC=C2)C(=O)NC)C=C1)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
90
CELSIUS
8
HOUR
A mixture containing 4-amino-3-nitrophenol 5 (1.0 g, 6.4 mmol), potassium bis(trimethylsilyl)amide (2.58 g, 12.8mmol) was stirred in DMF (50 ml) for 2 hours at rt. To this mixture was added (4-chloro(2-pyridyl))-N-methylcarboxamide 4 (1.09 g, 6.4 mmol) and potassium carbonate (0.5 g, 7.6 mmol) and stirred at 90° C. ove...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccncc1
c1ccncc1
c1ccncc1.c1ccccc1
HCl
CN(C)C=O
90
8
CNC(=O)c1cc(Cl)ccn1.Nc1ccc(O)cc1[N+](=O)[O-]>CN(C)C=O>CNC(=O)c1cc(Oc2ccc(N)c([N+](=O)[O-])c2)ccn1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ab655c226c6f4bdaa38913a1d9d27f6d
Cn1c(Nc2ccc(Cl)cc2)nc2cc(Oc3ccnc(C#N)c3)ccc21.NCCN>>Cn1c(Nc2ccc(Cl)cc2)nc2cc(Oc3ccnc(C4=NCCN4)c3)ccc21
OS(=O)(=O)O.ClC1=CC=C(C=C1)NC1=NC2=C(N1C)C=CC(=C2)OC2=CC(=NC=C2)C#N.C(CN)N>>ClC1=CC=C(C=C1)NC1=NC2=C(N1C)C=CC(=C2)OC2=CC(=NC=C2)C=2NCCN2
[CH3:1][n:2]1[c:3]([NH:4][c:5]2[cH:6][cH:7][c:8]([Cl:9])[cH:10][cH:11]2)[n:12][c:13]2[cH:14][c:15]([O:16][c:17]3[cH:18][cH:19][n:20][c:21]([C:22]#[N:23])[cH:27]3)[cH:28][cH:29][c:30]12.N[CH2:24][CH2:25][NH2:26]>>[CH3:1][n:2]1[c:3]([NH:4][c:5]2[cH:6][cH:7][c:8]([Cl:9])[cH:10][cH:11]2)[n:12][c:13]2[cH:14][c:15]([O:16][c:...
Cn1c(Nc2ccc(Cl)cc2)nc2cc(Oc3ccnc(C#N)c3)ccc21.NCCN
Cn1c(Nc2ccc(Cl)cc2)nc2cc(Oc3ccnc(C4=NCCN4)c3)ccc21
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
44acbf70f9cc2ac0a229971bc6e7c77034e28fcd162de6449941e21cd576fef7
e5ee524a9b0e5a2fe21766a24b1795b0d2b08a43f7dda8289a0ee59c7b4777e1
c1ccc(Nc2nc3cc(Oc4ccnc(C5=NCCN5)c4)ccc3[nH]2)cc1
N-[CH2;D2;+0:1]-[C:2]-[NH2;D1;+0:3].[N;H0;D1;+0:4]#[C;H0;D2;+0:5]-[c:6](:[c:7]):[#7;a:8]:[c:9]>>[c:9]:[#7;a:8]:[c:6](-[C;H0;D3;+0:5]1=[N;H0;D2;+0:4]-[CH2;D2;+0:1]-[C:2]-[NH;D2;+0:3]-1):[c:7]
null
[]
null
null
72
HOUR
H2SO4 (454 mg) was added cautiously to a suspension of 4-[2-(4-chloro-phenylamino)-1-methyl-1H-benzoimidazol-5-yloxy]-pyridine-2-carbonitrile (60.0 mg) in ethylenediamine (0.50 mL). The system was shaken at room temperature for 72 hrs, then poured onto ice/NaHCO3. The solid product was collected, washed (H2O) air-dried...
10.6084/m9.figshare.5104873.v1
null
Nitrile.Primary amine.Primary amine
Secondary amine
null
C1=NCCN1
c1ccccc1.c1ccc2[nH]cnc2c1.c1ccncc1.C1=NCCN1
Other
null
null
72
Cn1c(Nc2ccc(Cl)cc2)nc2cc(Oc3ccnc(C#N)c3)ccc21.NCCN>>Cn1c(Nc2ccc(Cl)cc2)nc2cc(Oc3ccnc(C4=NCCN4)c3)ccc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-1795322710d64a18827233237661e114
COc1ccc(O)c([N+](=O)[O-])c1>>COc1ccc(O)c(N)c1
COC1=CC(=C(C=C1)O)[N+](=O)[O-]>>NC1=C(C=CC(=C1)OC)O
O=[N+:9]([O-])[c:8]1[c:6]([OH:7])[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:10]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([OH:7])[c:8]([NH2:9])[cH:10]1
COc1ccc(O)c([N+](=O)[O-])c1
COc1ccc(O)c(N)c1
null
[Pd]
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccccc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
The mixture containing 4-methoxy-2-nitrophenol in methanol with catalytic amount of 10% Pd/C was hydrogenated until disappearance of yellow color to yield 2-amino-4-methoxyphenol. MS: MH+=140. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1
Other
[Pd].CO
null
null
COc1ccc(O)c([N+](=O)[O-])c1>[Pd].CO>COc1ccc(O)c(N)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5bb9ac08edac4f298e8c88f6c4bce75c
CCOC(=S)S.COc1ccc(O)c(N)c1>>COc1ccc2oc(S)nc2c1
Cl.NC1=C(C=CC(=C1)OC)O.C(C)OC(=S)S.[K]>>COC=1C=CC2=C(N=C(O2)S)C1
CCO[C:8](S)=[S:9].[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([OH:7])[c:11]([NH2:10])[cH:12]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]2[o:7][c:8]([SH:9])[n:10][c:11]2[cH:12]1
CCOC(=S)S.COc1ccc(O)c(N)c1
COc1ccc2oc(S)nc2c1
null
null
N1=CC=CC=C1
Aromatic Heterocycle Formation
OtherReaction
cbd796ad84a3d0f4f6a7a8057a682577715ca2073711c8f8b817da9ab6bfd06c
823bc935aa85db31214f5df7ab28f890020dcca64ae332d898272b243d751e45
c1ccc2ocnc2c1
C-C-O-[C;H0;D3;+0:1](-S)=[S;H0;D1;+0:2].[NH2;D1;+0:3]-[c:4](:[c:5]):[c:6](-[OH;D1;+0:7]):[c:8]>>[SH;D1;+0:2]-[c;H0;D3;+0:1]1:[n;H0;D2;+0:3]:[c:4](:[c:5]):[c:6](:[c:8]):[o;H0;D2;+0:7]:1
null
[]
null
null
null
null
The mixture containing 2-amino-4-methoxyphenol(1 eq) and O-ethylxanthic acid, potassium salt (1.1 eq) in pyridine was refluxed for two hours. The resultant mixture was poured in to ice/water containing hydrochloric acid to yield a 5-methoxybenzoxazole-2-thiol as a tan solid. MS: MH+=182 Conditions: See reaction.notes.p...
10.6084/m9.figshare.5104873.v1
null
Ether.Aromatic alcohol.Primary amine.Thiocarbonyl
Aromatic thiol
c1ccccc1
c1ccc2ocnc2c1
c1ccc2ocnc2c1
Other
N1=CC=CC=C1
null
null
CCOC(=S)S.COc1ccc(O)c(N)c1>N1=CC=CC=C1>COc1ccc2oc(S)nc2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-2e97f87fdbdf42edaf1ff767056716ef
COc1ccc2oc(S)nc2c1.O=S(Cl)Cl>>COc1ccc2oc(Cl)nc2c1
COC=1C=CC2=C(N=C(O2)S)C1.CN(C)C=O.S(=O)(Cl)Cl>>ClC=1OC2=C(N1)C=C(C=C2)OC
S[c:8]1[o:7][c:6]2[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:12][c:11]2[n:10]1.O=S(Cl)[Cl:9]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]2[o:7][c:8]([Cl:9])[n:10][c:11]2[cH:12]1
COc1ccc2oc(S)nc2c1.O=S(Cl)Cl
COc1ccc2oc(Cl)nc2c1
null
null
null
Functional Group Interconversion
OtherReaction
1c41bf5098d22e1f88c8b16e9d2c9e06b431e9e2ad47b4751567995db94396e2
a58f0859c9c497bf36b64745c3cc5a524c946cefa35cff91cc1283f5fe2c360f
c1ccc2ocnc2c1
Cl-S(=O)-[Cl;H0;D1;+0:1].S-[c;H0;D3;+0:2]1:[#7;a:3]:[c:4]:[c:5]:[#8;a:6]:1>>[Cl;H0;D1;+0:1]-[c;H0;D3;+0:2]1:[#7;a:3]:[c:4]:[c:5]:[#8;a:6]:1
null
[]
null
null
null
null
The mixture containing 5-methoxybenzoxazole-2-thiol was heated in thionyl chloride with a drop of DMF. The resultant mixture was concentrated and partitioned between ethyl acetate and water. The organic layer was washed with brine and dried and concentrated. Purification on a silica gel column gave 2-chloro-5-methoxybe...
10.6084/m9.figshare.5104873.v1
null
Aromatic thiol
Aromatic halide
c1ccc2ocnc2c1
c1ccc2ocnc2c1
c1ccc2ocnc2c1
HCl
null
null
null
COc1ccc2oc(S)nc2c1.O=S(Cl)Cl>>COc1ccc2oc(Cl)nc2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d46419144c4b457395c31c7c0a85f395
COc1ccc2oc(Cl)nc2c1.Nc1ccc(Br)cc1>>COc1ccc2oc(Nc3ccc(Br)cc3)nc2c1
ClC=1OC2=C(N1)C=C(C=C2)OC.BrC1=CC=C(N)C=C1.C(C)(C)N(CC)C(C)C>>BrC1=CC=C(C=C1)NC=1OC2=C(N1)C=C(C=C2)OC
Cl[c:8]1[o:7][c:6]2[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:19][c:18]2[n:17]1.[NH2:9][c:10]1[cH:11][cH:12][c:13]([Br:14])[cH:15][cH:16]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]2[o:7][c:8]([NH:9][c:10]3[cH:11][cH:12][c:13]([Br:14])[cH:15][cH:16]3)[n:17][c:18]2[cH:19]1
COc1ccc2oc(Cl)nc2c1.Nc1ccc(Br)cc1
COc1ccc2oc(Nc3ccc(Br)cc3)nc2c1
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
Goldberg coupling aryl amine-aryl chloride
56122dec6b9213d311e74462a865e17687f4178b6e2e5d6eb3cc0c5bc48da7a7
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(Nc2nc3ccccc3o2)cc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#8;a:5]:1.[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[c:8]:[c:7](-[NH;D2;+0:6]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[#8;a:5]:1):[c:9]
null
[]
null
null
null
null
The mixture containing 2-chloro-5-methoxybenzoxazole(1 eq), 4-bromoaniline (2 eq) and diisopropylethylamine was refluxed in dimethylformamide. The resultant mixture was concentrated and partitioned between ethyl acetate and water. The organic layer was washed with brine and dried. Purification on silica gel gave (4-bro...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ccc2ocnc2c1
c1ccc2ocnc2c1
c1ccc2ocnc2c1.c1ccccc1
HCl
CN(C=O)C
null
null
COc1ccc2oc(Cl)nc2c1.Nc1ccc(Br)cc1>CN(C=O)C>COc1ccc2oc(Nc3ccc(Br)cc3)nc2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-de00dfaa78694367b14596480705f5c0
COc1ccc2oc(Nc3ccc(Br)cc3)nc2c1>>Oc1ccc2oc(Nc3ccc(Br)cc3)nc2c1
BrC1=CC=C(C=C1)NC=1OC2=C(N1)C=C(C=C2)OC.Br>>BrC1=CC=C(C=C1)NC=1OC2=C(N1)C=C(C=C2)O
C[O:1][c:2]1[cH:3][cH:4][c:5]2[o:6][c:7]([NH:8][c:9]3[cH:10][cH:11][c:12]([Br:13])[cH:14][cH:15]3)[n:16][c:17]2[cH:18]1>>[OH:1][c:2]1[cH:3][cH:4][c:5]2[o:6][c:7]([NH:8][c:9]3[cH:10][cH:11][c:12]([Br:13])[cH:14][cH:15]3)[n:16][c:17]2[cH:18]1
COc1ccc2oc(Nc3ccc(Br)cc3)nc2c1
Oc1ccc2oc(Nc3ccc(Br)cc3)nc2c1
null
null
null
Deprotection
Cleavage of methoxy ethers to alcohols
c5320c7dfa4f544d4900efcae9b3262bf0d5286bcf39c86109232351f35b23d5
26a36596df80ec137b0e8087297418351c93c32819177f680675220622f215d4
c1ccc(Nc2nc3ccccc3o2)cc1
C-[O;H0;D2;+0:1]-[c:2](:[c:3]):[c:4]:[c:5]:[#7;a:6]>>[#7;a:6]:[c:5]:[c:4]:[c:2](-[OH;D1;+0:1]):[c:3]
null
[]
null
null
6
MINUTE
The mixture of (4-bromophenyl)(5-methoxybenzoxazol-2-yl)amine and hydrobromic acid (48%) was subjected to the microwave at 150° C. for 6 mins to yield 2-[(4-bromophenyl)amino]benzoxazol-5-ol. MS: MH+=305 Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Ether
Aromatic alcohol
null
null
c1ccc2ocnc2c1.c1ccccc1
Other
null
null
0.1
COc1ccc2oc(Nc3ccc(Br)cc3)nc2c1>>Oc1ccc2oc(Nc3ccc(Br)cc3)nc2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-045c50a29b284c05a2fc9504042be566
CNC(=O)c1cc(Cl)ccn1.Oc1ccc2oc(Nc3ccc(Br)cc3)nc2c1>>CNC(=O)c1cc(Oc2ccc3oc(Nc4ccc(Br)cc4)nc3c2)ccn1
BrC1=CC=C(C=C1)NC=1OC2=C(N1)C=C(C=C2)O.C[Si](C)(C)[N-][Si](C)(C)C.[K+].ClC1=CC(=NC=C1)C(=O)NC.C([O-])([O-])=O.[K+].[K+]>>BrC1=CC=C(C=C1)NC=1OC2=C(N1)C=C(C=C2)OC2=CC(=NC=C2)C(=O)NC
Cl[c:7]1[cH:6][c:5]([C:3]([NH:2][CH3:1])=[O:4])[n:28][cH:27][cH:26]1.[OH:8][c:9]1[cH:10][cH:11][c:12]2[o:13][c:14]([NH:15][c:16]3[cH:17][cH:18][c:19]([Br:20])[cH:21][cH:22]3)[n:23][c:24]2[cH:25]1>>[CH3:1][NH:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([O:8][c:9]2[cH:10][cH:11][c:12]3[o:13][c:14]([NH:15][c:16]4[cH:17][cH:18][c:19]...
CNC(=O)c1cc(Cl)ccn1.Oc1ccc2oc(Nc3ccc(Br)cc3)nc2c1
CNC(=O)c1cc(Oc2ccc3oc(Nc4ccc(Br)cc4)nc3c2)ccn1
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
99925b30dd2603ae575cba81b58435d015cd6b7267cf347380904f25833af5f2
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1ccc(Nc2nc3cc(Oc4ccncc4)ccc3o2)cc1
Cl-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[#7;a:4]:[c:5](-[C:6](-[#7:7])=[O;D1;H0:8]):[c:9]:1.[#7;a:10]:[c:11]:[c:12]:[c:13](-[OH;D1;+0:14]):[c:15]>>[#7:7]-[C:6](=[O;D1;H0:8])-[c:5]1:[#7;a:4]:[c:3]:[c:2]:[c;H0;D3;+0:1](-[O;H0;D2;+0:14]-[c:13](:[c:15]):[c:12]:[c:11]:[#7;a:10]):[c:9]:1
null
[]
null
null
null
null
The mixture containing 2-[(4-bromophenyl)amino]benzoxazol-5-ol (1 eq), potassium bis(trimethylsilyl)amide (4 eq), was stirred in dimethylformamide for 30 min at room temperature. To this mixture was added (4-chloro(2-pyridyl)-N-methyl-carboxamide (1 eq) and Potassium carbonate (1.2 eq) and microwaved for 6 mins at 150°...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccncc1
c1ccncc1
c1ccncc1.c1ccc2ocnc2c1.c1ccccc1
HCl
CN(C=O)C
null
null
CNC(=O)c1cc(Cl)ccn1.Oc1ccc2oc(Nc3ccc(Br)cc3)nc2c1>CN(C=O)C>CNC(=O)c1cc(Oc2ccc3oc(Nc4ccc(Br)cc4)nc3c2)ccn1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4deca450243547aba33d3679d2121b53
CN(C)c1ccc(Nc2nc3cc(OC4(C(=O)O)C=CC=CN4)ccc3n2C)cc1.NCCN1CCCC1>>CN(C)c1ccc(Nc2nc3cc(OC4(C5CCN(CCNC=O)C5)C=CC=CN4)ccc3n2C)cc1
CN(C1=CC=C(C=C1)NC1=NC2=C(N1C)C=CC(=C2)OC2(NC=CC=C2)C(=O)O)C.N1(CCCC1)CCN.CN(C)C(=[N+](C)C)ON1C2=C(C=CC=C2)N=N1.F[P-](F)(F)(F)(F)F.C(C)(C)N(C(C)C)CC>>CN(C1=CC=C(C=C1)NC1=NC2=C(N1C)C=CC(=C2)OC2(NC=CC=C2)C2CCN(C2)CCNC=O)C
O[C:23]([C:15]1([O:14][c:13]2[cH:12][c:11]3[n:10][c:9]([NH:8][c:7]4[cH:6][cH:5][c:4]([N:2]([CH3:1])[CH3:3])[cH:37][cH:36]4)[n:34]([CH3:35])[c:33]3[cH:32][cH:31]2)[CH:26]=[CH:27][CH:28]=[CH:29][NH:30]1)=[O:24].[CH2:16]1[CH2:17][CH2:18][N:19]([CH2:20][CH2:21][NH2:22])[CH2:25]1>>[CH3:1][N:2]([CH3:3])[c:4]1[cH:5][cH:6][c:7...
CN(C)c1ccc(Nc2nc3cc(OC4(C(=O)O)C=CC=CN4)ccc3n2C)cc1.NCCN1CCCC1
CN(C)c1ccc(Nc2nc3cc(OC4(C5CCN(CCNC=O)C5)C=CC=CN4)ccc3n2C)cc1
null
null
O1CCCC1
Acylation
OtherReaction
a5e50ac5b0783937f71374bd54d64dcd468b1cd9c3c46ff2fd13ac1969cb495f
25b89026811e1b3313674b1746d98ae7463bb6ef1893abcfeee44f8692f48a05
C1=CNC(Oc2ccc3[nH]c(Nc4ccccc4)nc3c2)(C2CCNC2)C=C1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C;H0;D4;+0:3]1(-[#8:4]-[c:5])-[#7:6]-[C:7]=[C:8]-[C:9]=[C:10]-1.[NH2;D1;+0:11]-[C:12]-[C:13]-[#7:14]1-[C:15]-[C:16]-[CH2;D2;+0:17]-[C:18]-1>>[O;D1;H0:2]=[CH;D2;+0:1]-[NH;D2;+0:11]-[C:12]-[C:13]-[#7:14]1-[C:15]-[C:16]-[CH;D3;+0:17](-[C;H0;D4;+0:3]2(-[#8:4]-[c:5])-[#7:6]-[C:7]=[C:8]-[C:9]=...
null
[]
null
null
16
HOUR
To 4-(2-{[4-(dimethylamino)pheylamino)-1-methylbenzimidazol-5-yloxy)-pyridine-2-carboxylic acid (1 eq) in tetrahydrofuran was added 2-pyrrolidinylethylamine (2 eq), HBTU (2 eq) and N,N-diisopropylethylamine (4 eq) and stir at ambient temperature for 16 h. The mixture was then concentrated and partitioned between ethyl ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Ether.Primary amine
Ether.Secondary amide
C1=CCNC=C1.C1CC[NH]C1
C1CC[NH]C1.C1=CCNC=C1
c1ccccc1.c1ccc2nc[nH]c2c1.C1CC[NH]C1.C1=CCNC=C1
HO-
O1CCCC1
null
16
CN(C)c1ccc(Nc2nc3cc(OC4(C(=O)O)C=CC=CN4)ccc3n2C)cc1.NCCN1CCCC1>O1CCCC1>CN(C)c1ccc(Nc2nc3cc(OC4(C5CCN(CCNC=O)C5)C=CC=CN4)ccc3n2C)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-cf605cf541c748bcbfd63433e029fcd1
CNc1ccc(Oc2ccnc(C(=O)OC(C)(C)C)c2)cc1N.Cc1cc(Nc2nc3cc(Oc4ccnc(C(=O)OC(C)(C)C)c4)ccc3n2C)ccc1Br>>Cc1cc(Nc2nc3cc(OC4(C(=O)O)C=CC=CN4)ccc3n2C)ccc1Br
C(C)(C)(C)OC(=O)C1=NC=CC(=C1)OC1=CC2=C(N(C(=N2)NC2=CC(=C(C=C2)Br)C)C)C=C1.C(C)(C)(C)OC(=O)C1=NC=CC(=C1)OC1=CC(=C(C=C1)NC)N.NC(=S)N.FC(C(=O)O)(F)F.IC>>BrC1=C(C=C(C=C1)NC1=NC2=C(N1C)C=CC(=C2)OC2(NC=CC=C2)C(=O)O)C
CNc1ccc(O[c:17]2[cH:16][c:12]([C:13](=[O:14])[O:15]C(C)(C)C)[n:20][cH:19][cH:18]2)cc1N.CC(C)(C)OC(=O)c1cc([O:11][c:10]2[cH:9][c:8]3[n:7][c:6]([NH:5][c:4]4[cH:3][c:2]([CH3:1])[c:28]([Br:29])[cH:27][cH:26]4)[n:24]([CH3:25])[c:23]3[cH:22][cH:21]2)ccn1>>[CH3:1][c:2]1[cH:3][c:4]([NH:5][c:6]2[n:7][c:8]3[cH:9][c:10]([O:11][C:...
CNc1ccc(Oc2ccnc(C(=O)OC(C)(C)C)c2)cc1N.Cc1cc(Nc2nc3cc(Oc4ccnc(C(=O)OC(C)(C)C)c4)ccc3n2C)ccc1Br
Cc1cc(Nc2nc3cc(OC4(C(=O)O)C=CC=CN4)ccc3n2C)ccc1Br
null
null
C(Cl)Cl.CO
Heteroatom Alkylation and Arylation
OtherReaction
c651282c0e9166458f7bf44c3131d44357e2ab966df1308b03eb64c1632e1461
927c5677be0d03bc697f830bd5a0b340e77c09e60abf567ee55f389e8726ded4
C1=CNC(Oc2ccc3[nH]c(Nc4ccccc4)nc3c2)C=C1
C-C(-C)(-C)-O-C(=O)-c1:c:c(-[O;H0;D2;+0:1]-[c:2](:[c:3]):[c:4]:[c:5]:[#7;a:6]):c:c:n:1.C-N-c1:c:c:c(-O-[c;H0;D3;+0:7]2:[cH;D2;+0:8]:[c;H0;D3;+0:9](-[C:10](=[O;D1;H0:11])-[O;H0;D2;+0:12]-C(-C)(-C)-C):[n;H0;D2;+0:13]:[cH;D2;+0:14]:[cH;D2;+0:15]:2):c:c:1-N>>[#7;a:6]:[c:5]:[c:4]:[c:2](-[O;H0;D2;+0:1]-[C;H0;D4;+0:9]1(-[C:10...
null
[]
null
null
16
HOUR
To tert-butyl4-[3-amino-4-(methylamino)phenoxy]pyridine-2-carboxylate (1 eq) in methanol was added 4-bromo-3-methylbenzeneisothiocyanate (1 eq) and stir at ambient temperature for 16 h. Formation of the corresponding thiourea was followed by LC/MS. To it was then added iodomethane (1 eq) and heated to 60° C. for 2 h. F...
10.6084/m9.figshare.5104873.v1
null
Ester.Ester.Ether.Ether.Primary amine.Secondary amine.Boc.Boc
Enamine.Carboxylic acid.Ether.Conjugated diene
c1ccccc1.c1ccncc1.c1ccncc1
C1=CCNC=C1
c1ccccc1.c1ccc2nc[nH]c2c1.C1=CCNC=C1
HO-
C(Cl)Cl.CO
null
16
CNc1ccc(Oc2ccnc(C(=O)OC(C)(C)C)c2)cc1N.Cc1cc(Nc2nc3cc(Oc4ccnc(C(=O)OC(C)(C)C)c4)ccc3n2C)ccc1Br>C(Cl)Cl.CO>Cc1cc(Nc2nc3cc(OC4(C(=O)O)C=CC=CN4)ccc3n2C)ccc1Br
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-2068fbf5dc2e43fc95b2bf9dcc748188
Cc1cc(Nc2nc3cc(OC4(C(=O)O)C=CC=CN4)ccc3n2C)ccc1Br.NCCN1CCCC1>>Cc1cc(Nc2nc3cc(OC4(C5CCN(CCNC=O)C5)C=CC=CN4)ccc3n2C)ccc1Br
BrC1=C(C=C(C=C1)NC1=NC2=C(N1C)C=CC(=C2)OC2(NC=CC=C2)C(=O)O)C.N1(CCCC1)CCN.CN(C)C(=[N+](C)C)ON1C2=C(C=CC=C2)N=N1.F[P-](F)(F)(F)(F)F.C(C)(C)N(C(C)C)CC>>BrC1=C(C=C(C=C1)NC1=NC2=C(N1C)C=CC(=C2)OC2(NC=CC=C2)C2CCN(C2)CCNC=O)C
O[C:20]([C:12]1([O:11][c:10]2[cH:9][c:8]3[n:7][c:6]([NH:5][c:4]4[cH:3][c:2]([CH3:1])[c:35]([Br:36])[cH:34][cH:33]4)[n:31]([CH3:32])[c:30]3[cH:29][cH:28]2)[CH:23]=[CH:24][CH:25]=[CH:26][NH:27]1)=[O:21].[CH2:13]1[CH2:14][CH2:15][N:16]([CH2:17][CH2:18][NH2:19])[CH2:22]1>>[CH3:1][c:2]1[cH:3][c:4]([NH:5][c:6]2[n:7][c:8]3[cH...
Cc1cc(Nc2nc3cc(OC4(C(=O)O)C=CC=CN4)ccc3n2C)ccc1Br.NCCN1CCCC1
Cc1cc(Nc2nc3cc(OC4(C5CCN(CCNC=O)C5)C=CC=CN4)ccc3n2C)ccc1Br
null
null
O1CCCC1
Acylation
OtherReaction
a5e50ac5b0783937f71374bd54d64dcd468b1cd9c3c46ff2fd13ac1969cb495f
25b89026811e1b3313674b1746d98ae7463bb6ef1893abcfeee44f8692f48a05
C1=CNC(Oc2ccc3[nH]c(Nc4ccccc4)nc3c2)(C2CCNC2)C=C1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C;H0;D4;+0:3]1(-[#8:4]-[c:5])-[#7:6]-[C:7]=[C:8]-[C:9]=[C:10]-1.[NH2;D1;+0:11]-[C:12]-[C:13]-[#7:14]1-[C:15]-[C:16]-[CH2;D2;+0:17]-[C:18]-1>>[O;D1;H0:2]=[CH;D2;+0:1]-[NH;D2;+0:11]-[C:12]-[C:13]-[#7:14]1-[C:15]-[C:16]-[CH;D3;+0:17](-[C;H0;D4;+0:3]2(-[#8:4]-[c:5])-[#7:6]-[C:7]=[C:8]-[C:9]=...
null
[]
null
null
16
HOUR
To 4-(2-{[4-bromo-3-methylpheylamino)-1-methylbenzimidazol-5-yloxy)-pyridine-2-carboxylic acid(1 eq) in tetrahydrofuran was added 2-pyrrolidinylethylamine (2 eq), HBTU (2 eq) and N,N-diisopropylethylamine (4 eq) and stir at ambient temperature for 16 h. The mixture was then concentrated and partitioned between ethyl ac...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Ether.Primary amine
Ether.Secondary amide
C1=CCNC=C1.C1CC[NH]C1
C1CC[NH]C1.C1=CCNC=C1
c1ccccc1.c1ccc2nc[nH]c2c1.C1CC[NH]C1.C1=CCNC=C1
HO-
O1CCCC1
null
16
Cc1cc(Nc2nc3cc(OC4(C(=O)O)C=CC=CN4)ccc3n2C)ccc1Br.NCCN1CCCC1>O1CCCC1>Cc1cc(Nc2nc3cc(OC4(C5CCN(CCNC=O)C5)C=CC=CN4)ccc3n2C)ccc1Br
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-77af987f401e431faa61513a30c385ce
CNc1ccc(Oc2ccnc(C(=O)OC(C)(C)C)c2)cc1N.Cn1c(Nc2cc(C(F)(F)F)ccc2F)nc2cc(Oc3ccnc(C(=O)OC(C)(C)C)c3)ccc21.NC(N)=S>>Cn1c(Nc2cc(C(F)(F)F)ccc2F)nc2cc(OC3(C(=O)O)C=CC=CN3)ccc21
C(C)(C)(C)OC(=O)C1=NC=CC(=C1)OC1=CC2=C(N(C(=N2)NC2=C(C=CC(=C2)C(F)(F)F)F)C)C=C1.C(C)(C)(C)OC(=O)C1=NC=CC(=C1)OC1=CC(=C(C=C1)NC)N.NC(=S)N.FC(C(=O)O)(F)F.IC>>FC1=C(C=C(C=C1)C(F)(F)F)NC1=NC2=C(N1C)C=CC(=C2)OC2(NC=CC=C2)C(=O)O
CNc1ccc(Oc2ccnc([C:22](=[O:23])[O:24]C(C)(C)C)c2)cc1N.CC(C)(C)OC(=O)[c:26]1n[cH:28][cH:27][c:21]([O:20][c:19]2[cH:18][c:17]3[n:16][c:3]([NH:4][c:5]4[cH:6][c:7]([C:8]([F:9])([F:10])[F:11])[cH:12][cH:13][c:14]4[F:15])[n:2]([CH3:1])[c:32]3[cH:31][cH:30]2)[cH:25]1.NC(=S)[NH2:29]>>[CH3:1][n:2]1[c:3]([NH:4][c:5]2[cH:6][c:7](...
CNc1ccc(Oc2ccnc(C(=O)OC(C)(C)C)c2)cc1N.Cn1c(Nc2cc(C(F)(F)F)ccc2F)nc2cc(Oc3ccnc(C(=O)OC(C)(C)C)c3)ccc21.NC(N)=S
Cn1c(Nc2cc(C(F)(F)F)ccc2F)nc2cc(OC3(C(=O)O)C=CC=CN3)ccc21
null
null
C(Cl)Cl.CO
C-C Coupling
OtherReaction
aea9c54fe4921815ac01c46586f27cf72b719e60f75bcb23786d01b4869c9824
67ed9599112c34fcf96cf445349b3d87559530f619170487474df0344ae446d4
C1=CNC(Oc2ccc3[nH]c(Nc4ccccc4)nc3c2)C=C1
C-C(-C)(-C)-O-C(=O)-[c;H0;D3;+0:1]1:[cH;D2;+0:2]:[c;H0;D3;+0:3](-[#8:4]-[c:5]):[cH;D2;+0:6]:[cH;D2;+0:7]:n:1.C-N-c1:c:c:c(-O-c2:c:c:n:c(-[C;H0;D3;+0:8](=[O;D1;H0:9])-[O;H0;D2;+0:10]-C(-C)(-C)-C):c:2):c:c:1-N.N-C(=S)-[NH2;D1;+0:11]>>[O;D1;H0:9]=[C;H0;D3;+0:8](-[OH;D1;+0:10])-[C;H0;D4;+0:3]1(-[#8:4]-[c:5])-[CH;D2;+0:2]=[...
null
[]
null
null
16
HOUR
To tert-butyl4-[3-amino-4-(methylamino)phenoxy]pyridine-2-carboxylate (1 eq) in methanol was added 2-fluro-5-(trifluromethyl)benzeneisothiocyanate (1 eq) and stir at ambient temperature for 16 h. Formation of the corresponding thiourea was followed by LC/MS. To it was then added iodomethane (1 eq) and heated to 60° C. ...
10.6084/m9.figshare.5104873.v1
null
Ester.Ester.Ether.Ether.Thiourea.Primary amine.Secondary amine.Boc.Boc
Enamine.Carboxylic acid.Ether.Conjugated diene
c1ccccc1.c1ccncc1.c1ccncc1
C1=CCNC=C1
c1ccccc1.c1ccc2[nH]cnc2c1.C1=CCNC=C1
Other
C(Cl)Cl.CO
null
16
CNc1ccc(Oc2ccnc(C(=O)OC(C)(C)C)c2)cc1N.Cn1c(Nc2cc(C(F)(F)F)ccc2F)nc2cc(Oc3ccnc(C(=O)OC(C)(C)C)c3)ccc21.NC(N)=S>C(Cl)Cl.CO>Cn1c(Nc2cc(C(F)(F)F)ccc2F)nc2cc(OC3(C(=O)O)C=CC=CN3)ccc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c3fb996c828a4d13bda2ab66d028f62d
Cn1c(Nc2cc(C(F)(F)F)ccc2F)nc2cc(OC3(C(=O)O)C=CC=CN3)ccc21.NCCN1CCCC1>>Cn1c(Nc2cc(C(F)(F)F)ccc2F)nc2cc(OC3(C4CCN(CCNC=O)C4)C=CC=CN3)ccc21
FC1=C(C=C(C=C1)C(F)(F)F)NC1=NC2=C(N1C)C=CC(=C2)OC2(NC=CC=C2)C(=O)O.N1(CCCC1)CCN.CN(C)C(=[N+](C)C)ON1C2=C(C=CC=C2)N=N1.F[P-](F)(F)(F)(F)F.C(C)(C)N(C(C)C)CC>>FC1=C(C=C(C=C1)C(F)(F)F)NC1=NC2=C(N1C)C=CC(=C2)OC2(NC=CC=C2)C2CCN(C2)CCNC=O
O[C:29]([C:21]1([O:20][c:19]2[cH:18][c:17]3[n:16][c:3]([NH:4][c:5]4[cH:6][c:7]([C:8]([F:9])([F:10])[F:11])[cH:12][cH:13][c:14]4[F:15])[n:2]([CH3:1])[c:39]3[cH:38][cH:37]2)[CH:32]=[CH:33][CH:34]=[CH:35][NH:36]1)=[O:30].[CH2:22]1[CH2:23][CH2:24][N:25]([CH2:26][CH2:27][NH2:28])[CH2:31]1>>[CH3:1][n:2]1[c:3]([NH:4][c:5]2[cH...
Cn1c(Nc2cc(C(F)(F)F)ccc2F)nc2cc(OC3(C(=O)O)C=CC=CN3)ccc21.NCCN1CCCC1
Cn1c(Nc2cc(C(F)(F)F)ccc2F)nc2cc(OC3(C4CCN(CCNC=O)C4)C=CC=CN3)ccc21
null
null
O1CCCC1
Acylation
OtherReaction
a5e50ac5b0783937f71374bd54d64dcd468b1cd9c3c46ff2fd13ac1969cb495f
25b89026811e1b3313674b1746d98ae7463bb6ef1893abcfeee44f8692f48a05
C1=CNC(Oc2ccc3[nH]c(Nc4ccccc4)nc3c2)(C2CCNC2)C=C1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C;H0;D4;+0:3]1(-[#8:4]-[c:5])-[#7:6]-[C:7]=[C:8]-[C:9]=[C:10]-1.[NH2;D1;+0:11]-[C:12]-[C:13]-[#7:14]1-[C:15]-[C:16]-[CH2;D2;+0:17]-[C:18]-1>>[O;D1;H0:2]=[CH;D2;+0:1]-[NH;D2;+0:11]-[C:12]-[C:13]-[#7:14]1-[C:15]-[C:16]-[CH;D3;+0:17](-[C;H0;D4;+0:3]2(-[#8:4]-[c:5])-[#7:6]-[C:7]=[C:8]-[C:9]=...
null
[]
null
null
16
HOUR
To 4-(2-{[2-fluro-5-(trifluromethyl)phenylamino)-1-methylbenzimidazol-5-yl-oxy)pyridine-2-carboxylic acid (1 eq) in tetrahydrofuran was added 2-pyrrolidinylethylamine (2 eq), HBTU (2 eq) and N,N-diisopropylethylamine (4 eq) and stir at ambient temperature for 16 h. The mixture was then concentrated and partitioned betw...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Ether.Primary amine
Ether.Secondary amide
C1=CCNC=C1.C1CC[NH]C1
C1CC[NH]C1.C1=CCNC=C1
c1ccccc1.c1ccc2[nH]cnc2c1.C1CC[NH]C1.C1=CCNC=C1
HO-
O1CCCC1
null
16
Cn1c(Nc2cc(C(F)(F)F)ccc2F)nc2cc(OC3(C(=O)O)C=CC=CN3)ccc21.NCCN1CCCC1>O1CCCC1>Cn1c(Nc2cc(C(F)(F)F)ccc2F)nc2cc(OC3(C4CCN(CCNC=O)C4)C=CC=CN3)ccc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5e06cd34c97e405ab21ba84324b39d71
CNc1ccc(Oc2ccnc(C(=O)OC(C)(C)C)c2)cc1N.Cn1c(Nc2ccc(Br)c(F)c2)nc2cc(Oc3ccnc(C(=O)OC(C)(C)C)c3)ccc21>>Cn1c(Nc2ccc(Br)c(F)c2)nc2cc(OC3(C(=O)O)C=CC=CN3)ccc21
C(C)(C)(C)OC(=O)C1=NC=CC(=C1)OC1=CC2=C(N(C(=N2)NC2=CC(=C(C=C2)Br)F)C)C=C1.C(C)(C)(C)OC(=O)C1=NC=CC(=C1)OC1=CC(=C(C=C1)NC)N.NC(=S)N.FC(C(=O)O)(F)F.IC>>BrC1=C(C=C(C=C1)NC1=NC2=C(N1C)C=CC(=C2)OC2(NC=CC=C2)C(=O)O)F
CNc1ccc(Oc2cc([C:19](=[O:20])[O:21]C(C)(C)C)[n:26][cH:25][cH:24]2)cc1N.CC(C)(C)OC(=O)[c:23]1ncc[c:18]([O:17][c:16]2[cH:15][c:14]3[n:13][c:3]([NH:4][c:5]4[cH:6][cH:7][c:8]([Br:9])[c:10]([F:11])[cH:12]4)[n:2]([CH3:1])[c:29]3[cH:28][cH:27]2)[cH:22]1>>[CH3:1][n:2]1[c:3]([NH:4][c:5]2[cH:6][cH:7][c:8]([Br:9])[c:10]([F:11])[c...
CNc1ccc(Oc2ccnc(C(=O)OC(C)(C)C)c2)cc1N.Cn1c(Nc2ccc(Br)c(F)c2)nc2cc(Oc3ccnc(C(=O)OC(C)(C)C)c3)ccc21
Cn1c(Nc2ccc(Br)c(F)c2)nc2cc(OC3(C(=O)O)C=CC=CN3)ccc21
null
null
C(Cl)Cl.CO
C-C Coupling
OtherReaction
69f76c3b8a2300e5b27a5f67d2c164aa6431c7e55762dde8b548912e55721d5b
4edbc5aa10c177b20f61383c702da22155b87866fa39db7fef23ed8b6baa10fc
C1=CNC(Oc2ccc3[nH]c(Nc4ccccc4)nc3c2)C=C1
C-C(-C)(-C)-O-C(=O)-[c;H0;D3;+0:1]1:[cH;D2;+0:2]:[c;H0;D3;+0:3](-[#8:4]-[c:5]):c:c:n:1.C-N-c1:c:c:c(-O-c2:[cH;D2;+0:6]:[cH;D2;+0:7]:[n;H0;D2;+0:8]:c(-[C;H0;D3;+0:9](=[O;D1;H0:10])-[O;H0;D2;+0:11]-C(-C)(-C)-C):c:2):c:c:1-N>>[O;D1;H0:10]=[C;H0;D3;+0:9](-[OH;D1;+0:11])-[C;H0;D4;+0:3]1(-[#8:4]-[c:5])-[CH;D2;+0:2]=[CH;D2;+0...
null
[]
null
null
16
HOUR
To tert-butyl4-[3-amino-4-(methylamino)phenoxy]pyridine-2-carboxylate (1 eq) in methanol was added 4-bromo-3-flurobenzeneisothiocyanate (1 eq) and stir at ambient temperature for 16 h. Formation of the corresponding thiourea was followed by LC/MS. To it was then added iodomethane (1 eq) and heated to 60° C. for 2 h. Fo...
10.6084/m9.figshare.5104873.v1
null
Ester.Ester.Ether.Ether.Primary amine.Secondary amine.Boc.Boc
Enamine.Carboxylic acid.Ether.Conjugated diene
c1ccccc1.c1ccncc1.c1ccncc1
C1=CCNC=C1
c1ccccc1.c1ccc2[nH]cnc2c1.C1=CCNC=C1
HO-
C(Cl)Cl.CO
null
16
CNc1ccc(Oc2ccnc(C(=O)OC(C)(C)C)c2)cc1N.Cn1c(Nc2ccc(Br)c(F)c2)nc2cc(Oc3ccnc(C(=O)OC(C)(C)C)c3)ccc21>C(Cl)Cl.CO>Cn1c(Nc2ccc(Br)c(F)c2)nc2cc(OC3(C(=O)O)C=CC=CN3)ccc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-091680e93d774347987231f23e16a93f
Cn1c(Nc2ccc(Br)c(F)c2)nc2cc(OC3(C(=O)O)C=CC=CN3)ccc21.NCCC1CCCCN1>>Cn1c(Nc2ccc(Br)c(F)c2)nc2cc(OC3(C4CCNC(CCNC=O)C4)C=CC=CN3)ccc21
BrC1=C(C=C(C=C1)NC1=NC2=C(N1C)C=CC(=C2)OC2(NC=CC=C2)C(=O)O)F.N1C(CCCC1)CCN.CN(C)C(=[N+](C)C)ON1C2=C(C=CC=C2)N=N1.F[P-](F)(F)(F)(F)F.C(C)(C)N(C(C)C)CC>>BrC1=C(C=C(C=C1)NC1=NC2=C(N1C)C=CC(=C2)OC2(NC=CC=C2)C2CC(NCC2)CCNC=O)F
O[C:27]([C:18]1([O:17][c:16]2[cH:15][c:14]3[n:13][c:3]([NH:4][c:5]4[cH:6][cH:7][c:8]([Br:9])[c:10]([F:11])[cH:12]4)[n:2]([CH3:1])[c:37]3[cH:36][cH:35]2)[CH:30]=[CH:31][CH:32]=[CH:33][NH:34]1)=[O:28].[CH2:19]1[CH2:20][CH2:21][NH:22][CH:23]([CH2:24][CH2:25][NH2:26])[CH2:29]1>>[CH3:1][n:2]1[c:3]([NH:4][c:5]2[cH:6][cH:7][c...
Cn1c(Nc2ccc(Br)c(F)c2)nc2cc(OC3(C(=O)O)C=CC=CN3)ccc21.NCCC1CCCCN1
Cn1c(Nc2ccc(Br)c(F)c2)nc2cc(OC3(C4CCNC(CCNC=O)C4)C=CC=CN3)ccc21
null
null
O1CCCC1
Acylation
OtherReaction
bf1a936de3976a9cfd7abaadcadfdba07ae9915b3d8a8e69219619eaa53c3590
25b89026811e1b3313674b1746d98ae7463bb6ef1893abcfeee44f8692f48a05
C1=CNC(Oc2ccc3[nH]c(Nc4ccccc4)nc3c2)(C2CCNCC2)C=C1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C;H0;D4;+0:3]1(-[#8:4]-[c:5])-[#7:6]-[C:7]=[C:8]-[C:9]=[C:10]-1.[NH2;D1;+0:11]-[C:12]-[C:13]-[C:14]1-[#7:15]-[C:16]-[C:17]-[CH2;D2;+0:18]-[C:19]-1>>[O;D1;H0:2]=[CH;D2;+0:1]-[NH;D2;+0:11]-[C:12]-[C:13]-[C:14]1-[#7:15]-[C:16]-[C:17]-[CH;D3;+0:18](-[C;H0;D4;+0:3]2(-[#8:4]-[c:5])-[#7:6]-[C:7...
null
[]
null
null
16
HOUR
To 4-(2-{[4-bromo-3-fluropheylamino)-1-methylbenzimidazol-5-yloxy)pyridine-2-carboxylic acid (1 eq) in tetrahydrofuran was added 2-piperidylethylamine (2 eq), HBTU (2 eq) and N,N-diisopropylethylamine (4 eq) and stir at ambient temperature for 16 h. The mixture was then concentrated and partitioned between ethyl acetat...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Ether.Primary amine
Ether.Secondary amide
C1=CCNC=C1.C1CCNCC1
C1CCNCC1.C1=CCNC=C1
c1ccccc1.c1ccc2[nH]cnc2c1.C1CCNCC1.C1=CCNC=C1
HO-
O1CCCC1
null
16
Cn1c(Nc2ccc(Br)c(F)c2)nc2cc(OC3(C(=O)O)C=CC=CN3)ccc21.NCCC1CCCCN1>O1CCCC1>Cn1c(Nc2ccc(Br)c(F)c2)nc2cc(OC3(C4CCNC(CCNC=O)C4)C=CC=CN3)ccc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e34ada74913c4bee92a02dcdd4f03e69
CCc1ccc(Nc2nc3cc(Oc4ccnc(C(=O)OC(C)(C)C)c4)ccc3n2C)cc1>>CCc1ccc(Nc2nc3cc(OC4(C(=O)O)C=CC=CN4)ccc3n2C)cc1
C(C)(C)(C)OC(=O)C1=NC=CC(=C1)OC1=CC2=C(N(C(=N2)NC2=CC=C(C=C2)CC)C)C=C1.C(C)(C)(C)OC(=O)C1=NC=CC(=C1)OC1=CC(=C(C=C1)NC)N.NC(=S)N.FC(C(=O)O)(F)F.IC>>C(C)C1=CC=C(C=C1)NC1=NC2=C(N1C)C=CC(=C2)OC2(NC=CC=C2)C(=O)O
CC(C)(C)[O:17][C:15]([c:14]1[cH:18][c:19]([O:13][c:12]2[cH:11][c:10]3[n:9][c:8]([NH:7][c:6]4[cH:5][cH:4][c:3]([CH2:2][CH3:1])[cH:29][cH:28]4)[n:26]([CH3:27])[c:25]3[cH:24][cH:23]2)[cH:20][cH:21][n:22]1)=[O:16]>>[CH3:1][CH2:2][c:3]1[cH:4][cH:5][c:6]([NH:7][c:8]2[n:9][c:10]3[cH:11][c:12]([O:13][C:14]4([C:15](=[O:16])[OH:...
CCc1ccc(Nc2nc3cc(Oc4ccnc(C(=O)OC(C)(C)C)c4)ccc3n2C)cc1
CCc1ccc(Nc2nc3cc(OC4(C(=O)O)C=CC=CN4)ccc3n2C)cc1
null
null
C(Cl)Cl.CO
Reduction
OtherReaction
d3267c8cc68d2a5b89c3e6e8fab69387f9d7531c9843a66c036bcfaf2a30fb80
7af9e23356bd0e70bec1bc13ad619ccc3e02b9df9ac8a03ecfeb09c23c86c19e
C1=CNC(Oc2ccc3[nH]c(Nc4ccccc4)nc3c2)C=C1
C-C(-C)(-C)-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c;H0;D3;+0:4]1:[cH;D2;+0:5]:[c;H0;D3;+0:6](-[O;H0;D2;+0:7]-[c:8](:[c:9]):[c:10]:[c:11]:[#7;a:12]):[cH;D2;+0:13]:[cH;D2;+0:14]:[n;H0;D2;+0:15]:1>>[#7;a:12]:[c:11]:[c:10]:[c:8](-[O;H0;D2;+0:7]-[C;H0;D4;+0:4]1(-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1])-[CH;D2;+0:5]=[CH;D2;+0:6]-[CH;...
null
[]
null
null
16
HOUR
To tert-butyl4-[3-amino-4-(methylamino)phenoxy]pyridine-2-carboxylate (1 eq) in methanol was added 4-ethylbenzeneisothiocyanate (1 eq) and stir at ambient temperature for 16 h. Formation of the corresponding thiourea was followed by LC/MS. To it was then added iodomethane (1 eq) and heated to 60° C. for 2 h. Formation ...
10.6084/m9.figshare.5104873.v1
null
Ester.Ether.Boc
Enamine.Carboxylic acid.Ether.Conjugated diene
c1ccncc1
C1=CCNC=C1
c1ccccc1.c1ccc2nc[nH]c2c1.C1=CCNC=C1
Other
C(Cl)Cl.CO
null
16
CCc1ccc(Nc2nc3cc(Oc4ccnc(C(=O)OC(C)(C)C)c4)ccc3n2C)cc1>C(Cl)Cl.CO>CCc1ccc(Nc2nc3cc(OC4(C(=O)O)C=CC=CN4)ccc3n2C)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-6fb29f1c20dc42d685c70611cd0567a6
CCc1ccc(Nc2nc3cc(Oc4ccnc(C(=O)O)c4)ccc3n2C)cc1.NCCN1CCCC1>>CCc1ccc(Nc2nc3cc(OC4(C5CCN(CCNC=O)C5)C=CC=CN4)ccc3n2C)cc1
C(C)C1=CC=C(C=C1)NC1=NC2=C(N1C)C=CC(=C2)OC2=CC(=NC=C2)C(=O)O.N1(CCCC1)CCN.CN(C)C(=[N+](C)C)ON1C2=C(C=CC=C2)N=N1.F[P-](F)(F)(F)(F)F.C(C)(C)N(C(C)C)CC>>C(C)C1=CC=C(C=C1)NC1=NC2=C(N1C)C=CC(=C2)OC2(NC=CC=C2)C2CCN(C2)CCNC=O
O[C:22](=[O:23])[c:26]1[cH:25][c:14]([O:13][c:12]2[cH:11][c:10]3[n:9][c:8]([NH:7][c:6]4[cH:5][cH:4][c:3]([CH2:2][CH3:1])[cH:36][cH:35]4)[n:33]([CH3:34])[c:32]3[cH:31][cH:30]2)[cH:27][cH:28][n:29]1.[CH2:15]1[CH2:16][CH2:17][N:18]([CH2:19][CH2:20][NH2:21])[CH2:24]1>>[CH3:1][CH2:2][c:3]1[cH:4][cH:5][c:6]([NH:7][c:8]2[n:9]...
CCc1ccc(Nc2nc3cc(Oc4ccnc(C(=O)O)c4)ccc3n2C)cc1.NCCN1CCCC1
CCc1ccc(Nc2nc3cc(OC4(C5CCN(CCNC=O)C5)C=CC=CN4)ccc3n2C)cc1
null
null
O1CCCC1
Acylation
OtherReaction
43c7c99d7b02bd3a4807c6f78ebd3df0228169d9aeb5e4dde71257220982421b
1deae815888eed473c5335f3c03e53789c06dcbb831fcceb524365d2bc97aa94
C1=CNC(Oc2ccc3[nH]c(Nc4ccccc4)nc3c2)(C2CCNC2)C=C1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c;H0;D3;+0:3]1:[cH;D2;+0:4]:[c;H0;D3;+0:5](-[#8:6]-[c:7]):[cH;D2;+0:8]:[cH;D2;+0:9]:[n;H0;D2;+0:10]:1.[NH2;D1;+0:11]-[C:12]-[C:13]-[#7:14]1-[C:15]-[C:16]-[CH2;D2;+0:17]-[C:18]-1>>[O;D1;H0:2]=[CH;D2;+0:1]-[NH;D2;+0:11]-[C:12]-[C:13]-[#7:14]1-[C:15]-[C:16]-[CH;D3;+0:17](-[C;H0;D4;+0:5]2(-[...
null
[]
null
null
16
HOUR
To 4-(2-{[4-ethylpheyl]amino)-1-methylbenzimidazol-5-yloxy)pyridine-2-carboxylic acid (1 eq) in tetrahydrofuran was added 2-pyrrolidinylethylamine (2 eq), HBTU (2 eq) and N,N-diisopropylethylamine (4 eq) and stir at ambient temperature for 16 h. The mixture was then concentrated and partitioned between ethyl acetate an...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Ether.Primary amine
Enamine.Ether.Secondary amide.Conjugated diene
c1ccncc1.C1CC[NH]C1
C1CC[NH]C1.C1=CCNC=C1
c1ccccc1.c1ccc2nc[nH]c2c1.C1CC[NH]C1.C1=CCNC=C1
Other
O1CCCC1
null
16
CCc1ccc(Nc2nc3cc(Oc4ccnc(C(=O)O)c4)ccc3n2C)cc1.NCCN1CCCC1>O1CCCC1>CCc1ccc(Nc2nc3cc(OC4(C5CCN(CCNC=O)C5)C=CC=CN4)ccc3n2C)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e07ae407e2ad4211b517156c3f50540b
CNc1ccc(Oc2ccnc(C(=O)OC(C)(C)C)c2)cc1N.Cn1c(Nc2cccc(C(C)(C)C)c2)nc2cc(Oc3ccnc(C(=O)OC(C)(C)C)c3)ccc21>>Cn1c(Nc2cccc(C(C)(C)C)c2)nc2cc(OC3(C(=O)O)C=CC=CN3)ccc21
C(C)(C)(C)OC(=O)C1=NC=CC(=C1)OC1=CC2=C(N(C(=N2)NC2=CC(=CC=C2)C(C)(C)C)C)C=C1.C(C)(C)(C)OC(=O)C1=NC=CC(=C1)OC1=CC(=C(C=C1)NC)N.NC(=S)N.FC(C(=O)O)(F)F.IC>>C(C)(C)(C)C=1C=C(C=CC1)NC1=NC2=C(N1C)C=CC(=C2)OC2(NC=CC=C2)C(=O)O
CNc1ccc(Oc2cc([C:21](=[O:22])[O:23]C(C)(C)C)[n:28][cH:27][cH:26]2)cc1N.CC(C)(C)OC(=O)[c:25]1ncc[c:20]([O:19][c:18]2[cH:17][c:16]3[n:15][c:3]([NH:4][c:5]4[cH:6][cH:7][cH:8][c:9]([C:10]([CH3:11])([CH3:12])[CH3:13])[cH:14]4)[n:2]([CH3:1])[c:31]3[cH:30][cH:29]2)[cH:24]1>>[CH3:1][n:2]1[c:3]([NH:4][c:5]2[cH:6][cH:7][cH:8][c:...
CNc1ccc(Oc2ccnc(C(=O)OC(C)(C)C)c2)cc1N.Cn1c(Nc2cccc(C(C)(C)C)c2)nc2cc(Oc3ccnc(C(=O)OC(C)(C)C)c3)ccc21
Cn1c(Nc2cccc(C(C)(C)C)c2)nc2cc(OC3(C(=O)O)C=CC=CN3)ccc21
null
null
C(Cl)Cl.CO
C-C Coupling
OtherReaction
69f76c3b8a2300e5b27a5f67d2c164aa6431c7e55762dde8b548912e55721d5b
4edbc5aa10c177b20f61383c702da22155b87866fa39db7fef23ed8b6baa10fc
C1=CNC(Oc2ccc3[nH]c(Nc4ccccc4)nc3c2)C=C1
C-C(-C)(-C)-O-C(=O)-[c;H0;D3;+0:1]1:[cH;D2;+0:2]:[c;H0;D3;+0:3](-[#8:4]-[c:5]):c:c:n:1.C-N-c1:c:c:c(-O-c2:[cH;D2;+0:6]:[cH;D2;+0:7]:[n;H0;D2;+0:8]:c(-[C;H0;D3;+0:9](=[O;D1;H0:10])-[O;H0;D2;+0:11]-C(-C)(-C)-C):c:2):c:c:1-N>>[O;D1;H0:10]=[C;H0;D3;+0:9](-[OH;D1;+0:11])-[C;H0;D4;+0:3]1(-[#8:4]-[c:5])-[CH;D2;+0:2]=[CH;D2;+0...
null
[]
null
null
16
HOUR
To tert-butyl4-[3-amino-4-(methylamino)phenoxy]pyridine-2-carboxylate (1 eq) in methanol was added 3-(tert-butyl)benzeneisothiocyanate (1 eq) and stir at ambient temperature for 16 h. Formation of the corresponding thiourea was followed by LC/MS. To it was then added iodomethane (1 eq) and heated to 60° C. for 2 h. For...
10.6084/m9.figshare.5104873.v1
null
Ester.Ester.Ether.Ether.Primary amine.Secondary amine.Boc.Boc
Enamine.Carboxylic acid.Ether.Conjugated diene
c1ccccc1.c1ccncc1.c1ccncc1
C1=CCNC=C1
c1ccccc1.c1ccc2[nH]cnc2c1.C1=CCNC=C1
HO-
C(Cl)Cl.CO
null
16
CNc1ccc(Oc2ccnc(C(=O)OC(C)(C)C)c2)cc1N.Cn1c(Nc2cccc(C(C)(C)C)c2)nc2cc(Oc3ccnc(C(=O)OC(C)(C)C)c3)ccc21>C(Cl)Cl.CO>Cn1c(Nc2cccc(C(C)(C)C)c2)nc2cc(OC3(C(=O)O)C=CC=CN3)ccc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-31884a28b2674f72abfb5151acc15a1a
Cn1c(Nc2cccc(C(C)(C)C)c2)nc2cc(OC3(C(=O)O)C=CC=CN3)ccc21.NCCC1CCCCN1>>Cn1c(Nc2cccc(C(C)(C)C)c2)nc2cc(OC3(C4CCNC(CCNC=O)C4)C=CC=CN3)ccc21
C(C)(C)(C)C=1C=C(C=CC1)NC1=NC2=C(N1C)C=CC(=C2)OC2(NC=CC=C2)C(=O)O.N1C(CCCC1)CCN.CN(C)C(=[N+](C)C)ON1C2=C(C=CC=C2)N=N1.F[P-](F)(F)(F)(F)F.C(C)(C)N(C(C)C)CC>>C(C)(C)(C)C=1C=C(C=CC1)NC1=NC2=C(N1C)C=CC(=C2)OC2(NC=CC=C2)C2CC(NCC2)CCNC=O
O[C:29]([C:20]1([O:19][c:18]2[cH:17][c:16]3[n:15][c:3]([NH:4][c:5]4[cH:6][cH:7][cH:8][c:9]([C:10]([CH3:11])([CH3:12])[CH3:13])[cH:14]4)[n:2]([CH3:1])[c:39]3[cH:38][cH:37]2)[CH:32]=[CH:33][CH:34]=[CH:35][NH:36]1)=[O:30].[CH2:21]1[CH2:22][CH2:23][NH:24][CH:25]([CH2:26][CH2:27][NH2:28])[CH2:31]1>>[CH3:1][n:2]1[c:3]([NH:4]...
Cn1c(Nc2cccc(C(C)(C)C)c2)nc2cc(OC3(C(=O)O)C=CC=CN3)ccc21.NCCC1CCCCN1
Cn1c(Nc2cccc(C(C)(C)C)c2)nc2cc(OC3(C4CCNC(CCNC=O)C4)C=CC=CN3)ccc21
null
null
O1CCCC1
Acylation
OtherReaction
bf1a936de3976a9cfd7abaadcadfdba07ae9915b3d8a8e69219619eaa53c3590
25b89026811e1b3313674b1746d98ae7463bb6ef1893abcfeee44f8692f48a05
C1=CNC(Oc2ccc3[nH]c(Nc4ccccc4)nc3c2)(C2CCNCC2)C=C1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C;H0;D4;+0:3]1(-[#8:4]-[c:5])-[#7:6]-[C:7]=[C:8]-[C:9]=[C:10]-1.[NH2;D1;+0:11]-[C:12]-[C:13]-[C:14]1-[#7:15]-[C:16]-[C:17]-[CH2;D2;+0:18]-[C:19]-1>>[O;D1;H0:2]=[CH;D2;+0:1]-[NH;D2;+0:11]-[C:12]-[C:13]-[C:14]1-[#7:15]-[C:16]-[C:17]-[CH;D3;+0:18](-[C;H0;D4;+0:3]2(-[#8:4]-[c:5])-[#7:6]-[C:7...
null
[]
null
null
16
HOUR
To 4-(2-{[3-(tert-butyl)phenylamino)-1-methylbenzimidazol-5-yloxy)pyridine-2-carboxylic acid (1 eq) in tetrahydrofuran was added 2-piperidylethylamine (2 eq), HBTU (2 eq) and N,N-diisopropylethylamine (4 eq) and stir at ambient temperature for 16 h. The mixture was then concentrated and partitioned between ethyl acetat...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Ether.Primary amine
Ether.Secondary amide
C1=CCNC=C1.C1CCNCC1
C1CCNCC1.C1=CCNC=C1
c1ccccc1.c1ccc2[nH]cnc2c1.C1CCNCC1.C1=CCNC=C1
HO-
O1CCCC1
null
16
Cn1c(Nc2cccc(C(C)(C)C)c2)nc2cc(OC3(C(=O)O)C=CC=CN3)ccc21.NCCC1CCCCN1>O1CCCC1>Cn1c(Nc2cccc(C(C)(C)C)c2)nc2cc(OC3(C4CCNC(CCNC=O)C4)C=CC=CN3)ccc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c8ae1da528ce40c6b1958b78eb9caaca
CNc1ccc(Oc2ccnc(C(=O)OC(C)(C)C)c2)cc1N.Cn1c(Nc2ccc(Cl)c(C(F)(F)F)c2)nc2cc(Oc3ccnc(C(=O)OC(C)(C)C)c3)ccc21>>Cn1c(Nc2ccc(Cl)c(C(F)(F)F)c2)nc2cc(OC3(C(=O)O)C=CC=CN3)ccc21
C(C)(C)(C)OC(=O)C1=NC=CC(=C1)OC1=CC2=C(N(C(=N2)NC2=CC(=C(C=C2)Cl)C(F)(F)F)C)C=C1.C(C)(C)(C)OC(=O)C1=NC=CC(=C1)OC1=CC(=C(C=C1)NC)N.NC(=S)N.FC(C(=O)O)(F)F.IC>>ClC1=C(C=C(C=C1)NC1=NC2=C(N1C)C=CC(=C2)OC2(NC=CC=C2)C(=O)O)C(F)(F)F
CNc1ccc(Oc2cc([C:22](=[O:23])[O:24]C(C)(C)C)[n:29][cH:28][cH:27]2)cc1N.CC(C)(C)OC(=O)[c:26]1ncc[c:21]([O:20][c:19]2[cH:18][c:17]3[n:16][c:3]([NH:4][c:5]4[cH:6][cH:7][c:8]([Cl:9])[c:10]([C:11]([F:12])([F:13])[F:14])[cH:15]4)[n:2]([CH3:1])[c:32]3[cH:31][cH:30]2)[cH:25]1>>[CH3:1][n:2]1[c:3]([NH:4][c:5]2[cH:6][cH:7][c:8]([...
CNc1ccc(Oc2ccnc(C(=O)OC(C)(C)C)c2)cc1N.Cn1c(Nc2ccc(Cl)c(C(F)(F)F)c2)nc2cc(Oc3ccnc(C(=O)OC(C)(C)C)c3)ccc21
Cn1c(Nc2ccc(Cl)c(C(F)(F)F)c2)nc2cc(OC3(C(=O)O)C=CC=CN3)ccc21
null
null
C(Cl)Cl.CO
C-C Coupling
OtherReaction
69f76c3b8a2300e5b27a5f67d2c164aa6431c7e55762dde8b548912e55721d5b
4edbc5aa10c177b20f61383c702da22155b87866fa39db7fef23ed8b6baa10fc
C1=CNC(Oc2ccc3[nH]c(Nc4ccccc4)nc3c2)C=C1
C-C(-C)(-C)-O-C(=O)-[c;H0;D3;+0:1]1:[cH;D2;+0:2]:[c;H0;D3;+0:3](-[#8:4]-[c:5]):c:c:n:1.C-N-c1:c:c:c(-O-c2:[cH;D2;+0:6]:[cH;D2;+0:7]:[n;H0;D2;+0:8]:c(-[C;H0;D3;+0:9](=[O;D1;H0:10])-[O;H0;D2;+0:11]-C(-C)(-C)-C):c:2):c:c:1-N>>[O;D1;H0:10]=[C;H0;D3;+0:9](-[OH;D1;+0:11])-[C;H0;D4;+0:3]1(-[#8:4]-[c:5])-[CH;D2;+0:2]=[CH;D2;+0...
null
[]
null
null
16
HOUR
To tert-butyl4-[3-amino-4-(methylamino)phenoxy]pyridine-2-carboxylate (1 eq) in methanol was added 4-chloro-3-(trifluromethyl)benzeneisothiocyanate (1 eq) and stir at ambient temperature for 16 h. Formation of the corresponding thiourea was followed by LC/MS. To it was then added iodomethane (1 eq) and heated to 60° C....
10.6084/m9.figshare.5104873.v1
null
Ester.Ester.Ether.Ether.Primary amine.Secondary amine.Boc.Boc
Enamine.Carboxylic acid.Ether.Conjugated diene
c1ccccc1.c1ccncc1.c1ccncc1
C1=CCNC=C1
c1ccccc1.c1ccc2[nH]cnc2c1.C1=CCNC=C1
HO-
C(Cl)Cl.CO
null
16
CNc1ccc(Oc2ccnc(C(=O)OC(C)(C)C)c2)cc1N.Cn1c(Nc2ccc(Cl)c(C(F)(F)F)c2)nc2cc(Oc3ccnc(C(=O)OC(C)(C)C)c3)ccc21>C(Cl)Cl.CO>Cn1c(Nc2ccc(Cl)c(C(F)(F)F)c2)nc2cc(OC3(C(=O)O)C=CC=CN3)ccc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0a79efa2b0854b679e5635cea251931d
CNC(=O)c1cc(Oc2ccc(NC)c(N)c2)ccn1.O=C(Cl)c1ccc(CCl)cc1>>CNC(=O)c1cc(Oc2ccc3c(c2)nc(NC(=O)c2ccc(CCl)cc2)n3C)ccn1
[S-]C#N.[Na+].ClCC1=CC=C(C(=O)Cl)C=C1.NC=1C=C(OC2=CC(=NC=C2)C(=O)NC)C=CC1NC.Cl.C(C)N=C=NCCCN(C)C>>ClCC1=CC=C(C=C1)C(=O)NC1=NC2=C(N1C)C=CC(=C2)OC2=CC(=NC=C2)C(=O)NC
[CH3:1][NH:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([O:8][c:9]2[cH:10][cH:11][c:12]([NH:28][CH3:29])[c:13]([NH2:15])[cH:14]2)[cH:30][cH:31][n:32]1.Cl[C:18](=[O:19])[c:20]1[cH:21][cH:22][c:23]([CH2:24][Cl:25])[cH:26][cH:27]1>>[CH3:1][NH:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([O:8][c:9]2[cH:10][cH:11][c:12]3[c:13]([cH:14]2)[n:15][c:16...
CNC(=O)c1cc(Oc2ccc(NC)c(N)c2)ccn1.O=C(Cl)c1ccc(CCl)cc1
CNC(=O)c1cc(Oc2ccc3c(c2)nc(NC(=O)c2ccc(CCl)cc2)n3C)ccn1
null
null
CC(=O)C
Aromatic Heterocycle Formation
OtherReaction
6007ce27c8fab5f5472c061eb36aa5e117a23e5c5c565f74ceb6415f1e4399f6
f9acae1c78587942b501ef34ad83c994b8601ae314b6fafb351abe1b05ec8565
O=C(Nc1nc2cc(Oc3ccncc3)ccc2[nH]1)c1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C;D1;H3:6]-[NH;D2;+0:7]-[c:8](:[c:9]):[c:10](-[NH2;D1;+0:11]):[c:12]>>[C;D1;H3:6]-[n;H0;D3;+0:7]1:[c:8](:[c:9]):[c:10](:[c:12]):[n;H0;D2;+0:11]:[c:13]:1-[#7:14]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
null
[]
null
null
16
HOUR
A solution of sodium thiocyanate (1 eq) in acetone was added slowly in to a solution of 4-(chloromethyl)benzoylchloride (1 eq) in acetone at 0° C. The mixture was then filtered in to a solution of {4-[3-amino-4-(methylamino)phenoxy](2-pyridyl)}-N-methylcarboxamide (1 eq) in acetone. Formation of N-acylthiourea was foll...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine.Secondary amine
Secondary amide
c1ccccc1
c1ccc2nc[nH]c2c1
c1ccncc1.c1ccc2nc[nH]c2c1.c1ccccc1
HCl
CC(=O)C
null
16
CNC(=O)c1cc(Oc2ccc(NC)c(N)c2)ccn1.O=C(Cl)c1ccc(CCl)cc1>CC(=O)C>CNC(=O)c1cc(Oc2ccc3c(c2)nc(NC(=O)c2ccc(CCl)cc2)n3C)ccn1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-07dd05e6ebd64ac0b8c02b2d0f84ec50
Clc1ccnc(Cl)n1.OB(O)c1cccnc1>>Clc1nccc(-c2cccnc2)n1
ClC1=NC=CC(=N1)Cl.N1=CC(=CC=C1)B(O)O.C([O-])([O-])=O.[Na+].[Na+]>>ClC1=NC=CC(=N1)C=1C=NC=CC1
Cl[c:6]1[cH:5][cH:4][n:3][c:2]([Cl:1])[n:13]1.OB(O)[c:7]1[cH:8][cH:9][cH:10][n:11][cH:12]1>>[Cl:1][c:2]1[n:3][cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][n:11][cH:12]2)[n:13]1
Clc1ccnc(Cl)n1.OB(O)c1cccnc1
Clc1nccc(-c2cccnc2)n1
null
[Pd](Cl)Cl.C1(=CC=CC=C1)P(C1=CC=CC=C1)[C-]1C=CC=C1.[C-]1(C=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.[Fe+2]
O1CCCC1.O
C-C Coupling
Suzuki coupling with boronic acids
51855f0568b0c9a2f03c51034f8881daa4aef477007bbafb8803ff38f26b4c50
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1cncc(-c2ccncn2)c1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](-[Cl;D1;H0:4]):[#7;a:5]:[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8]1:[c:9]:[#7;a:10]:[c:11]:[c:12]:[c:13]:1>>[Cl;D1;H0:4]-[c:3]1:[#7;a:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8]2:[c:9]:[#7;a:10]:[c:11]:[c:12]:[c:13]:2):[c:7]:[c:6]:[#7;a:5]:1
null
[]
60
CELSIUS
null
null
Nitrogen was bubbled through a solution of 2,4-dichloropyrimidine (1 eq) in tetrahydrofuran and water (3:1) for 0.5 h. Bis(diphenylphosphino)ferrocene Palladium(II)chloride (0.05 eq) followed by pyridine-3-boronic acid (1 eq) and sodium carbonate (3 eq) was added and the mixture was heated to 60° C. for 16 h under nitr...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1cncnc1.c1ccncc1
c1cncnc1.c1ccncc1
c1cncnc1.c1ccncc1
HCl.B
[Pd](Cl)Cl.C1(=CC=CC=C1)P(C1=CC=CC=C1)[C-]1C=CC=C1.[C-]1(C=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.[Fe+2].O1CCCC1.O
60
null
Clc1ccnc(Cl)n1.OB(O)c1cccnc1>[Pd](Cl)Cl.C1(=CC=CC=C1)P(C1=CC=CC=C1)[C-]1C=CC=C1.[C-]1(C=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.[Fe+2].O1CCCC1.O>Clc1nccc(-c2cccnc2)n1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-489fdd3767e74cdab1836ba0effdcde5
Clc1nccc(-c2cccnc2)n1.Nc1ccc(O)cc1[N+](=O)[O-]>>Nc1ccc(Oc2nccc(-c3cccnc3)n2)cc1[N+](=O)[O-]
NC1=C(C=C(C=C1)O)[N+](=O)[O-].ClC1=NC=CC(=N1)C=1C=NC=CC1>>[N+](=O)([O-])C1=C(C=CC(=C1)OC1=NC=CC(=N1)C=1C=NC=CC1)N
Cl[c:7]1[n:8][cH:9][cH:10][c:11](-[c:12]2[cH:13][cH:14][cH:15][n:16][cH:17]2)[n:18]1.[NH2:1][c:2]1[cH:3][cH:4][c:5]([OH:6])[cH:19][c:20]1[N+:21](=[O:22])[O-:23]>>[NH2:1][c:2]1[cH:3][cH:4][c:5]([O:6][c:7]2[n:8][cH:9][cH:10][c:11](-[c:12]3[cH:13][cH:14][cH:15][n:16][cH:17]3)[n:18]2)[cH:19][c:20]1[N+:21](=[O:22])[O-:23]
Clc1nccc(-c2cccnc2)n1.Nc1ccc(O)cc1[N+](=O)[O-]
Nc1ccc(Oc2nccc(-c3cccnc3)n2)cc1[N+](=O)[O-]
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
38da1e480b17968341fc50d07104da93d31f20765e3b36e5a0790cb6b1d88a10
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1ccc(Oc2nccc(-c3cccnc3)n2)cc1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[#7;a:4]:[c:5].[OH;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[c:3]:[#7;a:2]:[c;H0;D3;+0:1](-[O;H0;D2;+0:6]-[c:7](:[c:8]):[c:9]):[#7;a:4]:[c:5]
null
[]
null
null
null
null
A solution of 4-amino-3-nitro-phenol (1 eq) and 2-chloro-4-(3-pyridyl)pyrimidine (1 eq) in N,N-dimethylformamide was microwaved at 150° C. for 10 mins. The reaction mixture was partitioned between ethyl acetate and water. The organic layer was concentrated and purified on silica gel to yield 2-nitro-4-(4-(3-pyridyl)pyr...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1cncnc1
c1cncnc1
c1ccccc1.c1cncnc1.c1ccncc1
HCl
CN(C=O)C
null
null
Clc1nccc(-c2cccnc2)n1.Nc1ccc(O)cc1[N+](=O)[O-]>CN(C=O)C>Nc1ccc(Oc2nccc(-c3cccnc3)n2)cc1[N+](=O)[O-]
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a7fcc24149aa4eb08f3039f2959434d8
Nc1ccc(Oc2nccc(-c3cccnc3)n2)cc1[N+](=O)[O-]>>Nc1ccc(Oc2nccc(-c3cccnc3)n2)cc1N
[N+](=O)([O-])C1=C(C=CC(=C1)OC1=NC=CC(=N1)C=1C=NC=CC1)N>>N1=CC(=CC=C1)C1=NC(=NC=C1)OC=1C=C(C(=CC1)N)N
O=[N+:21]([O-])[c:20]1[c:2]([NH2:1])[cH:3][cH:4][c:5]([O:6][c:7]2[n:8][cH:9][cH:10][c:11](-[c:12]3[cH:13][cH:14][cH:15][n:16][cH:17]3)[n:18]2)[cH:19]1>>[NH2:1][c:2]1[cH:3][cH:4][c:5]([O:6][c:7]2[n:8][cH:9][cH:10][c:11](-[c:12]3[cH:13][cH:14][cH:15][n:16][cH:17]3)[n:18]2)[cH:19][c:20]1[NH2:21]
Nc1ccc(Oc2nccc(-c3cccnc3)n2)cc1[N+](=O)[O-]
Nc1ccc(Oc2nccc(-c3cccnc3)n2)cc1N
null
[Pd]
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc(Oc2nccc(-c3cccnc3)n2)cc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
The mixture containing 2-nitro-4-(4-(3-pyridyl)pyrimidin-2-yloxy)phenylamine in methanol with catalytic amount of 10% Pd/C was hydrogenated until disappearance of yellow color to yield 4-(4-(3-pyridyl)pyrimidin-2-yloxy)benzene-1,2-diamine. MS: MH+=279. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1.c1cncnc1.c1ccncc1
Other
[Pd].CO
null
null
Nc1ccc(Oc2nccc(-c3cccnc3)n2)cc1[N+](=O)[O-]>[Pd].CO>Nc1ccc(Oc2nccc(-c3cccnc3)n2)cc1N
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-084fb7b4da67426aa581b30a57eee387
Nc1ccc(Oc2nccc(-c3cccnc3)n2)cc1N.O=C(Cl)c1ccc(CCl)cc1>>O=C(Nc1nc2ccc(Oc3nccc(-c4cccnc4)n3)cc2[nH]1)c1ccc(CCl)cc1
[S-]C#N.[Na+].ClCC1=CC=C(C(=O)Cl)C=C1.N1=CC(=CC=C1)C1=NC(=NC=C1)OC=1C=C(C(=CC1)N)N.Cl.C(C)N=C=NCCCN(C)C>>ClCC1=CC=C(C=C1)C(=O)NC=1NC2=C(N1)C=CC(=C2)OC2=NC=CC(=N2)C=2C=NC=CC2
[NH2:5][c:6]1[cH:7][cH:8][c:9]([O:10][c:11]2[n:12][cH:13][cH:14][c:15](-[c:16]3[cH:17][cH:18][cH:19][n:20][cH:21]3)[n:22]2)[cH:23][c:24]1[NH2:25].Cl[C:2](=[O:1])[c:26]1[cH:27][cH:28][c:29]([CH2:30][Cl:31])[cH:32][cH:33]1>>[O:1]=[C:2]([NH:3][c:4]1[n:5][c:6]2[cH:7][cH:8][c:9]([O:10][c:11]3[n:12][cH:13][cH:14][c:15](-[c:1...
Nc1ccc(Oc2nccc(-c3cccnc3)n2)cc1N.O=C(Cl)c1ccc(CCl)cc1
O=C(Nc1nc2ccc(Oc3nccc(-c4cccnc4)n3)cc2[nH]1)c1ccc(CCl)cc1
null
null
CC(=O)C
Aromatic Heterocycle Formation
OtherReaction
84492309ebd88369b38543aed3a10403ecb24f9be5ac8e8d692194c41bfc42f5
e3e959b05bda8dad38bcefce5939efac6b07ca7f2b99a15789ad53e999a19964
O=C(Nc1nc2ccc(Oc3nccc(-c4cccnc4)n3)cc2[nH]1)c1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9](-[NH2;D1;+0:10]):[c:11]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[#7:12]-[c:13]1:[n;H0;D2;+0:10]:[c:9](:[c:11]):[c:7](:[c:8]):[nH;D2;+0:6]:1)-[c:3](:[c:4]):[c:5]
null
[]
null
null
16
HOUR
A solution of sodium thiocyanate (1 eq) in acetone was added slowly in to a solution of 4-(chloromethyl)benzoylchloride (1 eq) in acetone at 0° C. The mixture was then filtered in to a solution of 4-(4-(3-pyridyl)pyrimidin-2-yloxy)benzene-1,2-diamine (1 eq) in acetone. Formation of N-acylthiourea was followed by LC/MS....
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine.Primary amine
Secondary amide
c1ccccc1
c1ccc2[nH]cnc2c1
c1ccc2[nH]cnc2c1.c1cncnc1.c1ccncc1.c1ccccc1
HCl
CC(=O)C
null
16
Nc1ccc(Oc2nccc(-c3cccnc3)n2)cc1N.O=C(Cl)c1ccc(CCl)cc1>CC(=O)C>O=C(Nc1nc2ccc(Oc3nccc(-c4cccnc4)n3)cc2[nH]1)c1ccc(CCl)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b9a59be9cda948e58ac95e309bfa0a86
CCN1CCNCC1.O=[N+]([O-])c1ccc(F)cc1>>CCN1CCN(c2ccc([N+](=O)[O-])cc2)CC1
FC1=CC=C(C=C1)[N+](=O)[O-].C(C)N1CCNCC1.C(C)(C)N(C(C)C)CC>>C(C)N1CCN(CC1)C1=CC=C(C=C1)[N+](=O)[O-]
[CH3:1][CH2:2][N:3]1[CH2:4][CH2:5][NH:6][CH2:16][CH2:17]1.F[c:7]1[cH:8][cH:9][c:10]([N+:11](=[O:12])[O-:13])[cH:14][cH:15]1>>[CH3:1][CH2:2][N:3]1[CH2:4][CH2:5][N:6]([c:7]2[cH:8][cH:9][c:10]([N+:11](=[O:12])[O-:13])[cH:14][cH:15]2)[CH2:16][CH2:17]1
CCN1CCNCC1.O=[N+]([O-])c1ccc(F)cc1
CCN1CCN(c2ccc([N+](=O)[O-])cc2)CC1
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
Buchwald-Hartwig/Ullmann-Goldberg/N-arylation secondary amine
d687b31bdda9f407fdde6ca57e67eee0681e173646c617afef7770c56d05bab9
b6b8e2cdb45054a35f5e8157d624f852c0601a09401556706e166b19536eb7a7
c1ccc(N2CCNCC2)cc1
F-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[#7:6]1-[C:7]-[C:8]-[NH;D2;+0:9]-[C:10]-[C:11]-1>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[N;H0;D3;+0:9]1-[C:8]-[C:7]-[#7:6]-[C:11]-[C:10]-1):[c:4]:[c:5]
null
[]
80
CELSIUS
null
null
To 4-fluro-1-nitrobenzene(1 eq) in N,N-dimethylformamide was added Ethyl piperazine (2 eq) and N,N-diisopropylethyl amine (2 eq) and heated at 80° C. for 16 h. Concentrated the resultant mixture and partitioned between ethyl acetate and water. The organic layer was then washed with brine and dried with sodium sulfate a...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Secondary amine
Tertiary amine
C1C[NH]CCN1.c1ccccc1
C1C[NH]CC[NH]1.c1ccccc1
C1C[NH]CC[NH]1.c1ccccc1
HF
CN(C=O)C
80
null
CCN1CCNCC1.O=[N+]([O-])c1ccc(F)cc1>CN(C=O)C>CCN1CCN(c2ccc([N+](=O)[O-])cc2)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-81e578f4f7604e9c85bdfe9dfa76cfd4
CCN1CCN(c2ccc([N+](=O)[O-])cc2)CC1>>CCN1CCN(c2ccc(N)cc2)CC1
C(C)N1CCN(CC1)C1=CC=C(C=C1)[N+](=O)[O-]>>C(C)N1CCN(CC1)C1=CC=C(C=C1)N
O=[N+:11]([O-])[c:10]1[cH:9][cH:8][c:7]([N:6]2[CH2:5][CH2:4][N:3]([CH2:2][CH3:1])[CH2:15][CH2:14]2)[cH:13][cH:12]1>>[CH3:1][CH2:2][N:3]1[CH2:4][CH2:5][N:6]([c:7]2[cH:8][cH:9][c:10]([NH2:11])[cH:12][cH:13]2)[CH2:14][CH2:15]1
CCN1CCN(c2ccc([N+](=O)[O-])cc2)CC1
CCN1CCN(c2ccc(N)cc2)CC1
null
[Pd]
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc(N2CCNCC2)cc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
The mixture containing 4-ethyl-1-(4-nitrophenyl)piperazine in methanol with catalytic amount of 10% Pd/C was hydrogenated to yield 4-(4-ethylpiperazinyl)phenylamine. MS: MH+=205. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
C1C[NH]CC[NH]1.c1ccccc1
Other
[Pd].CO
null
null
CCN1CCN(c2ccc([N+](=O)[O-])cc2)CC1>[Pd].CO>CCN1CCN(c2ccc(N)cc2)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c9a54c6438a5492985c4aac36f9c2b88
C1COCCN1.O=[N+]([O-])c1ccc(CCBr)cc1>>O=[N+]([O-])c1ccc(CCN2CCOCC2)cc1
BrCCC1=CC=C(C=C1)[N+](=O)[O-].N1CCOCC1>>[N+](=O)([O-])C1=CC=C(C=C1)CCN1CCOCC1
[NH:10]1[CH2:11][CH2:12][O:13][CH2:14][CH2:15]1.Br[CH2:9][CH2:8][c:7]1[cH:6][cH:5][c:4]([N+:2](=[O:1])[O-:3])[cH:17][cH:16]1>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]([CH2:8][CH2:9][N:10]2[CH2:11][CH2:12][O:13][CH2:14][CH2:15]2)[cH:16][cH:17]1
C1COCCN1.O=[N+]([O-])c1ccc(CCBr)cc1
O=[N+]([O-])c1ccc(CCN2CCOCC2)cc1
null
null
O1CCCC1
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
2bad30dcdb0a20edb8ce877f072b133eedfd870621da393ec393128bfee00977
523d37155b42c8dc851abeddadebb241cdd90bdf649ba750c35e13c8c752d7b0
c1ccc(CCN2CCOCC2)cc1
Br-[CH2;D2;+0:1]-[C:2]-[c:3].[#8:4]1-[C:5]-[C:6]-[NH;D2;+0:7]-[C:8]-[C:9]-1>>[c:3]-[C:2]-[CH2;D2;+0:1]-[N;H0;D3;+0:7]1-[C:6]-[C:5]-[#8:4]-[C:9]-[C:8]-1
null
[]
null
null
16
HOUR
To 4-(2-bromoethyl)-1-nitrobenzene(1 eq) in tetrahydrofuran was added morpholine (3 eq) and stir for 16 h at ambient temperature. Concentrating and passing through a plug of silica gave 4-[2-(4-nitrophenyl)ethylmorpholine. MS: MH+=236. Conditions: See reaction.notes.procedure_details. Workup: Concentrating
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amine
Tertiary amine
C1COCCN1
C1COCC[NH]1
c1ccccc1.C1COCC[NH]1
HBr
O1CCCC1
null
16
C1COCCN1.O=[N+]([O-])c1ccc(CCBr)cc1>O1CCCC1>O=[N+]([O-])c1ccc(CCN2CCOCC2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ff93e64ab2394f70bb775a9f0729521e
O=[N+]([O-])c1ccc(CCN2CCOCC2)cc1>>Nc1ccc(CCN2CCOCC2)cc1
[N+](=O)([O-])C1=CC=C(C=C1)CCN1CCOCC1>>N1(CCOCC1)CCC1=CC=C(C=C1)N
O=[N+:1]([O-])[c:2]1[cH:3][cH:4][c:5]([CH2:6][CH2:7][N:8]2[CH2:9][CH2:10][O:11][CH2:12][CH2:13]2)[cH:14][cH:15]1>>[NH2:1][c:2]1[cH:3][cH:4][c:5]([CH2:6][CH2:7][N:8]2[CH2:9][CH2:10][O:11][CH2:12][CH2:13]2)[cH:14][cH:15]1
O=[N+]([O-])c1ccc(CCN2CCOCC2)cc1
Nc1ccc(CCN2CCOCC2)cc1
null
[Pd]
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc(CCN2CCOCC2)cc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
The mixture containing 4-[2-(4-nitrophenyl)ethyl]morpholine in methanol with catalytic amount of 10% Pd/C was hydrogenated to yield 4-(2-morpholin-4-ylethyl)phenylamine. MS: MH+=206. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1.C1COCC[NH]1
Other
[Pd].CO
null
null
O=[N+]([O-])c1ccc(CCN2CCOCC2)cc1>[Pd].CO>Nc1ccc(CCN2CCOCC2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-2ddcd16f5d4e40acba51d53f18999402
CC(=O)c1ccc([N+](=O)[O-])cc1.NCc1ccccc1>>O=[N+]([O-])c1ccc(CCNCc2ccccc2)cc1
[N+](=O)([O-])C1=CC=C(C=C1)C(C)=O.C1(=CC=CC=C1)CN.C(C)(=O)O[BH-](OC(C)=O)OC(C)=O.[Na+]>>[N+](=O)([O-])C1=CC=C(C=C1)CCNCC1=CC=CC=C1
O=[C:8]([c:7]1[cH:6][cH:5][c:4]([N+:2](=[O:1])[O-:3])[cH:19][cH:18]1)[CH3:9].[NH2:10][CH2:11][c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]([CH2:8][CH2:9][NH:10][CH2:11][c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[cH:18][cH:19]1
CC(=O)c1ccc([N+](=O)[O-])cc1.NCc1ccccc1
O=[N+]([O-])c1ccc(CCNCc2ccccc2)cc1
null
null
CO
Functional Group Addition
OtherReaction
19fd62cf2098e96a4130feef29e9bf81adb1ccfebe3387cc1f5e2935ebb7056f
b485541a30741fb92d734951552491c7748625ed3b5658b6b29d788a0e8f8e57
c1ccc(CCNCc2ccccc2)cc1
O=[C;H0;D3;+0:1](-[CH3;D1;+0:2])-[c:3](:[c:4]):[c:5].[NH2;D1;+0:6]-[C:7]-[c:8]>>[c:8]-[C:7]-[NH;D2;+0:6]-[CH2;D2;+0:2]-[CH2;D2;+0:1]-[c:3](:[c:4]):[c:5]
null
[]
null
null
16
HOUR
To a solution of 1-(4-nitrophenyl)ethan-1-one (1 eq) and phenylmethylamine (1 eq) in methanol was added sodiumtriacetoxyborohydride (1.2 eq). The resulting mixture was stirred at ambient temperature for 16 h. The mixture was concentrated and partitioned between ethyl acetate and water. The organic layer was concentrate...
10.6084/m9.figshare.5104873.v1
null
Ketone.Primary amine
Secondary amine
null
null
c1ccccc1.c1ccccc1
Other
CO
null
16
CC(=O)c1ccc([N+](=O)[O-])cc1.NCc1ccccc1>CO>O=[N+]([O-])c1ccc(CCNCc2ccccc2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-72aac1ae9609429b8f12400afb045713
O=[N+]([O-])c1ccc(CCNCc2ccccc2)cc1>>Nc1ccc(CCNCc2ccccc2)cc1
[N+](=O)([O-])C1=CC=C(C=C1)CCNCC1=CC=CC=C1>>NC1=CC=C(C=C1)CCNCC1=CC=CC=C1
O=[N+:1]([O-])[c:2]1[cH:3][cH:4][c:5]([CH2:6][CH2:7][NH:8][CH2:9][c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[cH:16][cH:17]1>>[NH2:1][c:2]1[cH:3][cH:4][c:5]([CH2:6][CH2:7][NH:8][CH2:9][c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[cH:16][cH:17]1
O=[N+]([O-])c1ccc(CCNCc2ccccc2)cc1
Nc1ccc(CCNCc2ccccc2)cc1
null
[Pd]
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc(CCNCc2ccccc2)cc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
The mixture containing [(4-nitrophenyl)ethyl]benzylamine in methanol with catalytic amount of 10% Pd/C was hydrogenated until disappearance of yellow color to yield [(4-aminophenyl)ethyl]benzylamine. MS: MH+=226. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1.c1ccccc1
Other
[Pd].CO
null
null
O=[N+]([O-])c1ccc(CCNCc2ccccc2)cc1>[Pd].CO>Nc1ccc(CCNCc2ccccc2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-2d2c569091a24068afd16715b91f3390
NC(=O)C(F)(F)F.Nc1cc(F)ccc1[N+](=O)[O-]>>NCc1cc(F)ccc1[N+](=O)[O-]
S(=O)(=O)(OC)OC.FC=1C=CC(=C(C1)N)[N+](=O)[O-].FC(C(=O)OC(C(F)(F)F)=O)(F)F.FC(C(=O)N)(F)F.[OH-].[Na+]>>FC=1C=CC(=C(C1)CN)[N+](=O)[O-]
O=[C:2](C(F)(F)F)[NH2:1].N[c:3]1[cH:4][c:5]([F:6])[cH:7][cH:8][c:9]1[N+:10](=[O:11])[O-:12]>>[NH2:1][CH2:2][c:3]1[cH:4][c:5]([F:6])[cH:7][cH:8][c:9]1[N+:10](=[O:11])[O-:12]
NC(=O)C(F)(F)F.Nc1cc(F)ccc1[N+](=O)[O-]
NCc1cc(F)ccc1[N+](=O)[O-]
null
[Cl-].C(C1=CC=CC=C1)[N+](C)(C)C
C(C)#N.C1(=CC=CC=C1)C.C(Cl)Cl
C-C Coupling
OtherReaction
57eeb6cb444d729ea25c9af40d90b2b85339cfcfa01a82f89f645f8d3327247a
c6562711aeb2bb6c0ed826650c3482d37ecfc2f4b0030c6f964c1758331569dd
c1ccccc1
F-C(-F)(-F)-[C;H0;D3;+0:1](=O)-[N;D1;H2:2].N-[c;H0;D3;+0:3](:[c:4]:[c:5]):[c:6](-[#7;+:7]):[c:8]>>[#7;+:7]-[c:6](:[c:8]):[c;H0;D3;+0:3](-[CH2;D2;+0:1]-[N;D1;H2:2]):[c:4]:[c:5]
null
[]
0
CELSIUS
10
MINUTE
A solution of 5-fluro-2-nitrophenylamine (1 eq) in methylenechloride was treated with trifluoroacetic anhydride (1 eq) and stirred for 10 minutes at 0° C. The mixture was quenched with saturated sodium bicarbonate solution. The organic layer was separated and washed with water, brine, dried and evaporated. To the solut...
10.6084/m9.figshare.5104873.v1
null
Trifluoro group.Primary amide.Primary amine
null
c1ccccc1
c1ccccc1
c1ccccc1
Other
[Cl-].C(C1=CC=CC=C1)[N+](C)(C)C.C(C)#N.C1(=CC=CC=C1)C.C(Cl)Cl
0
0.166667
NC(=O)C(F)(F)F.Nc1cc(F)ccc1[N+](=O)[O-]>[Cl-].C(C1=CC=CC=C1)[N+](C)(C)C.C(C)#N.C1(=CC=CC=C1)C.C(Cl)Cl>NCc1cc(F)ccc1[N+](=O)[O-]
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-40acfaf085a14c889f79846a72fdd46b
CN(C)C=O.CNC(=O)c1cccc(O)c1.C[Si](C)(C)[N-][Si](C)(C)C.Nc1cc(F)ccc1[N+](=O)[O-]>>CNC(=O)c1cc(Oc2ccc([N+](=O)[O-])c(NC)c2)ccn1
CN(C=O)C.FC=1C=CC(=C(C1)N)[N+](=O)[O-].C[Si](C)(C)[N-][Si](C)(C)C.[K+].OC=1C=C(C=CC1)C(=O)NC.C([O-])([O-])=O.[K+].[K+]>>CNC(=O)C1=NC=CC(=C1)OC1=CC(=C(C=C1)[N+](=O)[O-])NC
CN(C=O)[CH3:18].c1[c:5]([C:3]([NH:2][CH3:1])=[O:4])[cH:6][c:7]([OH:8])[cH:20][cH:21]1.C[Si](C)(C)[N-:22][Si](C)(C)C.F[c:9]1[cH:10][cH:11][c:12]([N+:13](=[O:14])[O-:15])[c:16]([NH2:17])[cH:19]1>>[CH3:1][NH:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([O:8][c:9]2[cH:10][cH:11][c:12]([N+:13](=[O:14])[O-:15])[c:16]([NH:17][CH3:18])[cH...
CN(C)C=O.CNC(=O)c1cccc(O)c1.C[Si](C)(C)[N-][Si](C)(C)C.Nc1cc(F)ccc1[N+](=O)[O-]
CNC(=O)c1cc(Oc2ccc([N+](=O)[O-])c(NC)c2)ccn1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
c634879a8d4528500fc2be3de37e4a0ee8d423d97c1d4f23bc31c4f4d8266e30
54c57484907ba531ad2d669934ec72f5a32e91a9ba1ac88e7bbfd9456582c8a2
c1ccc(Oc2ccncc2)cc1
C-N(-[CH3;D1;+0:1])-C=O.C-[Si](-C)(-C)-[N-;H0;D2:2]-[Si](-C)(-C)-C.F-[c;H0;D3;+0:3]1:[c:4]:[c:5]:[c:6]:[c:7](-[NH2;D1;+0:8]):[c:9]:1.[C;D1;H3:10]-[#7:11]-[C:12](=[O;D1;H0:13])-[c;H0;D3;+0:14]1:[c:15]:[c:16](-[OH;D1;+0:17]):[c:18]:[cH;D2;+0:19]:c:1>>[C;D1;H3:10]-[#7:11]-[C:12](=[O;D1;H0:13])-[c;H0;D3;+0:14]1:[c:15]:[c:1...
null
[]
90
CELSIUS
16
HOUR
The mixture containing 5-fluro-2-nitrophenylamine (1 eq), Potassium bis(trimethylsilyl)amide (2 eq) was stirred in dimethylformamide for 2 hours at room temperature. To this mixture was added (3-hydroxyphenyl)-N-methylcarboxamide (1 eq) and Potassium carbonate (1.2 eq) and stirred at 90° C. for 16 h. The reaction mixtu...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Tertiary amide.Aromatic alcohol.Primary amine.Silyl protective group.Silyl protective group
Ether.Secondary amine
c1ccccc1.c1ccccc1
c1ccncc1.c1ccccc1
c1ccncc1.c1ccccc1
HF
null
90
16
CN(C)C=O.CNC(=O)c1cccc(O)c1.C[Si](C)(C)[N-][Si](C)(C)C.Nc1cc(F)ccc1[N+](=O)[O-]>>CNC(=O)c1cc(Oc2ccc([N+](=O)[O-])c(NC)c2)ccn1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-204e0e7bf12a4fd99666168d14b4e1c1
CNC(=O)c1cc(Oc2ccc(N)c(NC)c2)ccn1.S=C=Nc1ccc(Br)cc1>>CNC(=O)c1cc(Oc2ccc3nc(Nc4ccc(Br)cc4)n(C)c3c2)ccn1
IC.NC1=C(C=C(OC2=CC(=NC=C2)C(=O)NC)C=C1)NC.BrC1=CC=C(C=C1)N=C=S>>BrC1=CC=C(C=C1)NC1=NC2=C(N1C)C=C(C=C2)OC2=CC(=NC=C2)C(=O)NC
[CH3:1][NH:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([O:8][c:9]2[cH:10][cH:11][c:12]([NH2:13])[c:25]([NH:23][CH3:24])[cH:26]2)[cH:27][cH:28][n:29]1.S=[C:14]=[N:15][c:16]1[cH:17][cH:18][c:19]([Br:20])[cH:21][cH:22]1>>[CH3:1][NH:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([O:8][c:9]2[cH:10][cH:11][c:12]3[n:13][c:14]([NH:15][c:16]4[cH:17][cH...
CNC(=O)c1cc(Oc2ccc(N)c(NC)c2)ccn1.S=C=Nc1ccc(Br)cc1
CNC(=O)c1cc(Oc2ccc3nc(Nc4ccc(Br)cc4)n(C)c3c2)ccn1
null
null
CO
Aromatic Heterocycle Formation
OtherReaction
4b3e260fa6094641dfa114b35f3471079a338332f41031b31ba4b7bb465b4139
c2745d0d96944794048cb0a435469fb3c0efa689f6d5e8d4fd6447372cabc5f8
c1ccc(Nc2nc3ccc(Oc4ccncc4)cc3[nH]2)cc1
S=[C;H0;D2;+0:1]=[N;H0;D2;+0:2]-[c:3](:[c:4]):[c:5].[C;D1;H3:6]-[NH;D2;+0:7]-[c:8](:[c:9]):[c:10](-[NH2;D1;+0:11]):[c:12]>>[C;D1;H3:6]-[n;H0;D3;+0:7]1:[c:8](:[c:9]):[c:10](:[c:12]):[n;H0;D2;+0:11]:[c;H0;D3;+0:1]:1-[NH;D2;+0:2]-[c:3](:[c:4]):[c:5]
null
[]
60
CELSIUS
2
HOUR
A solution of the {4-[4-amino-3-(methylamino)phenoxy](2-pyridyl)}-N-methyl-carboxamide(1 eq) in methanol was treated with 4-bromophenylisothiocyanate (1 eq) and stirred at 60° C. for 2 hours. The reaction mixture was cooled down to room temperature and iodomethane (1 eq) was added and stirred overnight at 60° C. The re...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Secondary amine.Isothiocyanate
Secondary amine
c1ccccc1
c1ccc2[nH]cnc2c1
c1ccncc1.c1ccc2[nH]cnc2c1.c1ccccc1
Other
CO
60
2
CNC(=O)c1cc(Oc2ccc(N)c(NC)c2)ccn1.S=C=Nc1ccc(Br)cc1>CO>CNC(=O)c1cc(Oc2ccc3nc(Nc4ccc(Br)cc4)n(C)c3c2)ccn1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b2672337f49f4fea831bf1a6c0ab6f63
Nc1ccc([N+](=O)[O-])cc1N.S=C=Nc1ccc(Br)cc1>>O=[N+]([O-])c1ccc2nc(Nc3ccc(Br)cc3)[nH]c2c1
IC.[N+](=O)([O-])C=1C=C(C(=CC1)N)N.BrC1=CC=C(C=C1)N=C=S>>BrC1=CC=C(C=C1)NC=1NC2=C(N1)C=CC(=C2)[N+](=O)[O-]
[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]([NH2:8])[c:19]([NH2:18])[cH:20]1.S=[C:9]=[N:10][c:11]1[cH:12][cH:13][c:14]([Br:15])[cH:16][cH:17]1>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][cH:6][c:7]2[n:8][c:9]([NH:10][c:11]3[cH:12][cH:13][c:14]([Br:15])[cH:16][cH:17]3)[nH:18][c:19]2[cH:20]1
Nc1ccc([N+](=O)[O-])cc1N.S=C=Nc1ccc(Br)cc1
O=[N+]([O-])c1ccc2nc(Nc3ccc(Br)cc3)[nH]c2c1
null
null
CO
Aromatic Heterocycle Formation
OtherReaction
b379a633a6d6a7ef71a4ec729ac27ffb0470b0a7feb5a79c5b4b49860868cf5b
85c21648c239f13e3de224b3880be5fbcc059dde8446f4822bf814f376b11c25
c1ccc(Nc2nc3ccccc3[nH]2)cc1
S=[C;H0;D2;+0:1]=[N;H0;D2;+0:2]-[c:3](:[c:4]):[c:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9](-[NH2;D1;+0:10]):[c:11]>>[c:4]:[c:3](-[NH;D2;+0:2]-[c;H0;D3;+0:1]1:[n;H0;D2;+0:10]:[c:9](:[c:11]):[c:7](:[c:8]):[nH;D2;+0:6]:1):[c:5]
null
[]
60
CELSIUS
2
HOUR
A solution of the 4-nitrobenzene-1,2-diamine in methanol was treated with 4-bromo phenyl isothiocyanate (1 eq) and stirred at 60° C. for 2 hours. The reaction mixture was cooled down to room temperature and iodomethane (1 eq) was added and stirred overnight at 60° C. The reaction was concentrated and purified on silica...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Primary amine.Isothiocyanate
Secondary amine
c1ccccc1
c1ccc2[nH]cnc2c1
c1ccc2[nH]cnc2c1.c1ccccc1
Other
CO
60
2
Nc1ccc([N+](=O)[O-])cc1N.S=C=Nc1ccc(Br)cc1>CO>O=[N+]([O-])c1ccc2nc(Nc3ccc(Br)cc3)[nH]c2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f7c4bbc0a17847169a23efc66b8dd681
CCN(CC)CC.CNC(=O)c1cc(Oc2ccc(N)c(N)c2)ccn1.O=C(O)Cc1ccc(Br)cc1>>CNC(=O)c1cc(Oc2ccc3c(c2)nc(Cc2ccc(Br)cc2)n3C)ccn1
BrC1=CC=C(C=C1)CC(=O)O.C(C(=O)Cl)(=O)Cl.NC=1C=C(OC2=CC(=NC=C2)C(=O)NC)C=CC1N.C(C)N(CC)CC>>BrC1=CC=C(C=C1)CC1=NC2=C(N1C)C=CC(=C2)OC2=CC(=NC=C2)C(=O)NC
CCN(CC)C[CH3:26].[CH3:1][NH:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([O:8][c:9]2[cH:10][cH:11][c:12]([NH2:25])[c:13]([NH2:15])[cH:14]2)[cH:27][cH:28][n:29]1.O=[C:16](O)[CH2:17][c:18]1[cH:19][cH:20][c:21]([Br:22])[cH:23][cH:24]1>>[CH3:1][NH:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([O:8][c:9]2[cH:10][cH:11][c:12]3[c:13]([cH:14]2)[n:15][...
CCN(CC)CC.CNC(=O)c1cc(Oc2ccc(N)c(N)c2)ccn1.O=C(O)Cc1ccc(Br)cc1
CNC(=O)c1cc(Oc2ccc3c(c2)nc(Cc2ccc(Br)cc2)n3C)ccn1
null
null
ClCCl.O1CCCC1.CN(C=O)C
Aromatic Heterocycle Formation
OtherReaction
7bb2feb927f3b80cd9b65f74956a8f03463f56769daffd1fb82b38e5a408a8b2
eb25e1adb2dda9b12f5be7597398e322af6c055fe8481cf7bc7c0f04aa065c68
c1ccc(Cc2nc3cc(Oc4ccncc4)ccc3[nH]2)cc1
C-C-N(-C-C)-C-[CH3;D1;+0:1].O-[C;H0;D3;+0:2](=O)-[C:3]-[c:4].[NH2;D1;+0:5]-[c:6](:[c:7]):[c:8](-[NH2;D1;+0:9]):[c:10]>>[CH3;D1;+0:1]-[n;H0;D3;+0:9]1:[c:8](:[c:10]):[c:6](:[c:7]):[n;H0;D2;+0:5]:[c;H0;D3;+0:2]:1-[C:3]-[c:4]
null
[]
60
CELSIUS
2
HOUR
To 4-bromophenyl acetic acid (1 eq) in dichoromethane containing a drop of N,N-dimethyl formamide at 0° C. was added oxalyl chloride (1.2 eq). The resulting mixture was then brought to ambient temperature and stirred for 2 h. The mixture was concentrated and to it was added tetrahydrofuran and [4-(3,4-diaminophenoxy)(2...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine.Primary amine.Tertiary amine
null
c1ccccc1
c1ccc2nc[nH]c2c1
c1ccncc1.c1ccc2nc[nH]c2c1.c1ccccc1
HO-
ClCCl.O1CCCC1.CN(C=O)C
60
2
CCN(CC)CC.CNC(=O)c1cc(Oc2ccc(N)c(N)c2)ccn1.O=C(O)Cc1ccc(Br)cc1>ClCCl.O1CCCC1.CN(C=O)C>CNC(=O)c1cc(Oc2ccc3c(c2)nc(Cc2ccc(Br)cc2)n3C)ccn1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4993b6bd45dd4b758422db41b7abca7f
O=C(O)c1ccc(N=C=S)cc1>>O=C(O)c1ccccc1
IC.NC=1C=C(OC2=CC(=NC=C2)C(=O)NC)C=CC1NC.N(=C=S)C1=CC=C(C(=O)O)C=C1>>C(C1=CC=CC=C1)(=O)O
S=C=N[c:7]1[cH:6][cH:5][c:4]([C:2](=[O:1])[OH:3])[cH:9][cH:8]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][cH:7][cH:8][cH:9]1
O=C(O)c1ccc(N=C=S)cc1
O=C(O)c1ccccc1
null
null
CO
Functional Group Interconversion
OtherReaction
9f8c98612863acf953fea7ac735cf5ef5c9344111235f882da4aeae8bee29c12
4e930e84ca7a4b5a1b2ffdfd0ad5173746b70455a6634f66996611a6644c2fb6
c1ccccc1
S=C=N-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]>>[c:3]:[c:2]:[cH;D2;+0:1]:[c:4]:[c:5]
null
[]
60
CELSIUS
3
HOUR
To {4-[3-amino-4-(methylamino)phenoxy](2-pyridyl)}-N-methylcarboxamide (1 eq) in methanol was added 4-isothiocyanatobenzoic acid (1 eq) and stirred at 60° C. for 3 h. To it was then added iodomethane (1 eq) and heated to 60° C. for 3 h. and concentrated the solvent and purified on silica gel to yield 4-({1-methyl-5-[2-...
10.6084/m9.figshare.5104873.v1
null
Isothiocyanate
null
c1ccccc1
c1ccccc1
c1ccccc1
Other
CO
60
3
O=C(O)c1ccc(N=C=S)cc1>CO>O=C(O)c1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-29296f4d1995470382504a5d3d73f23e
O=C(O)c1cccc(N=C=S)c1>>O=C(O)c1ccccc1
IC.CNC=O.N(=C=S)C=1C=C(C(=O)O)C=CC1>>C(C1=CC=CC=C1)(=O)O
S=C=N[c:6]1[cH:5][c:4]([C:2](=[O:1])[OH:3])[cH:9][cH:8][cH:7]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][cH:7][cH:8][cH:9]1
O=C(O)c1cccc(N=C=S)c1
O=C(O)c1ccccc1
null
null
CO
Functional Group Interconversion
OtherReaction
9f8c98612863acf953fea7ac735cf5ef5c9344111235f882da4aeae8bee29c12
4e930e84ca7a4b5a1b2ffdfd0ad5173746b70455a6634f66996611a6644c2fb6
c1ccccc1
S=C=N-[c;H0;D3;+0:1](:[c:2]:[c:3]-[C:4](=[O;D1;H0:5])-[O;D1;H1:6]):[c:7]:[c:8]>>[O;D1;H0:5]=[C:4](-[O;D1;H1:6])-[c:3]:[c:2]:[cH;D2;+0:1]:[c:7]:[c:8]
null
[]
60
CELSIUS
3
HOUR
To 4-[3-amino-4-(methylamino)phenoxy](2-pyridyl)}-N-methylcarboxamide (1 eq) in methanol was added 3-isothiocyanatobenzoic acid (1 eq) and stirred at 60° C. for 3 h. To it was then added iodomethane (1 eq) and heated to 60° C. for 3 h and concentrated the solvent and purified on silica gel to yield 3-({1-methyl-5-[2-(N...
10.6084/m9.figshare.5104873.v1
null
Isothiocyanate
null
c1ccccc1
c1ccccc1
c1ccccc1
Other
CO
60
3
O=C(O)c1cccc(N=C=S)c1>CO>O=C(O)c1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-7dedb8c1722640c2ab736f437c5820fd
CNC(=O)c1cccc(Cl)c1.CNc1cc(OC)c(O)cc1[N+](=O)[O-]>>CNC(=O)c1cc(Oc2cc([N+](=O)[O-])c(NC)cc2OC)ccn1
ClC=1C=C(C=CC1)C(=O)NC.C([O-])([O-])=O.[K+].[K+].COC1=C(C=C(C(=C1)NC)[N+](=O)[O-])O.CC(C)([O-])C.[K+].CN(C(C)=O)C>>COC1=C(OC2=CC(=NC=C2)C(=O)NC)C=C(C(=C1)NC)[N+](=O)[O-]
Cl[c:7]1[cH:6][c:5]([C:3]([NH:2][CH3:1])=[O:4])c[cH:23][cH:22]1.[OH:8][c:9]1[cH:10][c:11]([N+:12](=[O:13])[O-:14])[c:15]([NH:16][CH3:17])[cH:18][c:19]1[O:20][CH3:21]>>[CH3:1][NH:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([O:8][c:9]2[cH:10][c:11]([N+:12](=[O:13])[O-:14])[c:15]([NH:16][CH3:17])[cH:18][c:19]2[O:20][CH3:21])[cH:22][...
CNC(=O)c1cccc(Cl)c1.CNc1cc(OC)c(O)cc1[N+](=O)[O-]
CNC(=O)c1cc(Oc2cc([N+](=O)[O-])c(NC)cc2OC)ccn1
null
null
null
Protection
OtherReaction
f0023f5cb78e4f43639596fb9d7e792c21b5d63a2c4e24a596c544a93eb8f3cf
cf1075be1c1ecf3bb8058899ddc12870a38487ecc9322d6e66205e53a46d9b16
c1ccc(Oc2ccncc2)cc1
Cl-[c;H0;D3;+0:1]1:[c:2]:[cH;D2;+0:3]:c:[c;H0;D3;+0:4](-[C:5](=[O;D1;H0:6])-[#7:7]-[C;D1;H3:8]):[c:9]:1.[OH;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[C;D1;H3:8]-[#7:7]-[C:5](=[O;D1;H0:6])-[c;H0;D3;+0:4]1:[#7;a:14]:[cH;D2;+0:3]:[c:2]:[c;H0;D3;+0:1](-[O;H0;D2;+0:10]-[c:11](:[c:12]):[c:13]):[c:9]:1
null
[]
null
null
null
null
To a stirred solution of 2-methoxy-4-(methylamino)-5-nitrophenol(1 eq) in N,N-dimethylacetamide was added potassium-t-butoxide (1.2 eq) and continued stirring at ambient temperature until it solidified. To it was then added (3-chlorophenyl)-N-methylcarboxamide (1 eq) and anhydrous potassium carbonate (1 eq) and the res...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccccc1
c1ccncc1
c1ccncc1.c1ccccc1
HCl
null
null
null
CNC(=O)c1cccc(Cl)c1.CNc1cc(OC)c(O)cc1[N+](=O)[O-]>>CNC(=O)c1cc(Oc2cc([N+](=O)[O-])c(NC)cc2OC)ccn1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4060eb24e13c46d8965a91c2c6d0bd1f
CNc1cc(OC)c(Oc2ccnc(C(=O)OC(C)(C)C)c2)cc1N.Cn1c(Nc2ccc(Cl)cc2)nc2cc(Oc3ccnc(C(=O)OC(C)(C)C)c3)ccc21>>COc1cc2c(cc1OC1(C(=O)O)C=CC=CN1)nc(Nc1ccc(Cl)cc1)n2C
C(C)(C)(C)OC(=O)C1=NC=CC(=C1)OC1=CC2=C(N(C(=N2)NC2=CC=C(C=C2)Cl)C)C=C1.C(C)(C)(C)OC(=O)C1=NC=CC(=C1)OC1=CC(=C(C=C1OC)NC)N.NC(=S)N.FC(C(=O)O)(F)F.IC>>ClC1=CC=C(C=C1)NC1=NC2=C(N1C)C=C(C(=C2)OC2(NC=CC=C2)C(=O)O)OC
CNc1c(N)[cH:7][c:8]([O:9][c:10]2[cH:14][c:15]([C:11](=[O:12])[O:13]C(C)(C)C)[n:18][cH:17][cH:16]2)[c:3]([O:2][CH3:1])[cH:4]1.CC(C)(C)OC(=O)c1cc(Oc2cc[c:5]3[c:6](c2)[n:19][c:20]([NH:21][c:22]2[cH:23][cH:24][c:25]([Cl:26])[cH:27][cH:28]2)[n:29]3[CH3:30])ccn1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([cH:7][c:8]1[O:9][C:10]1([...
CNc1cc(OC)c(Oc2ccnc(C(=O)OC(C)(C)C)c2)cc1N.Cn1c(Nc2ccc(Cl)cc2)nc2cc(Oc3ccnc(C(=O)OC(C)(C)C)c3)ccc21
COc1cc2c(cc1OC1(C(=O)O)C=CC=CN1)nc(Nc1ccc(Cl)cc1)n2C
null
null
C(Cl)Cl.CO
C-C Coupling
OtherReaction
29efb81d47594bacad1863038bfbc6613a20e196cacf2349980ec228b88f5977
4edbc5aa10c177b20f61383c702da22155b87866fa39db7fef23ed8b6baa10fc
C1=CNC(Oc2ccc3[nH]c(Nc4ccccc4)nc3c2)C=C1
C-C(-C)(-C)-O-C(=O)-c1:c:c(-O-c2:c:c:[c;H0;D3;+0:1]3:[#7;a:2](-[C;D1;H3:3]):[c:4](-[#7:5]):[#7;a:6]:[c;H0;D3;+0:7]:3:c:2):c:c:n:1.C-N-c1:[cH;D2;+0:8]:[c:9](-[#8:10]):[c:11](-[#8:12]-[c;H0;D3;+0:13]2:[cH;D2;+0:14]:[c;H0;D3;+0:15](-[C;H0;D3;+0:16](=[O;D1;H0:17])-[O;H0;D2;+0:18]-C(-C)(-C)-C):[n;H0;D2;+0:19]:[cH;D2;+0:20]:...
null
[]
null
null
16
HOUR
To tert-butyl4-[3-amino-6-methoxy-4-(methylamino)phenoxy]pyridine-2-carboxylate(1 eq) in methanol was added 4-chlorobenzeneisothiocyanate (1 eq) and stir at ambient temperature for 16 h. Formation of the corresponding thiourea was followed by LC/MS. To it was then added iodomethane (1 eq) and heated to 60° C. for 2 h. ...
10.6084/m9.figshare.5104873.v1
null
Ester.Ester.Ether.Ether.Primary amine.Secondary amine.Boc.Boc
Enamine.Carboxylic acid.Ether.Conjugated diene
c1ccccc1.c1ccncc1.c1ccncc1.c1nc2ccccc2[nH]1
C1=CCNC=C1.c1ccc2[nH]cnc2c1
C1=CCNC=C1.c1ccc2[nH]cnc2c1.c1ccccc1
HO-
C(Cl)Cl.CO
null
16
CNc1cc(OC)c(Oc2ccnc(C(=O)OC(C)(C)C)c2)cc1N.Cn1c(Nc2ccc(Cl)cc2)nc2cc(Oc3ccnc(C(=O)OC(C)(C)C)c3)ccc21>C(Cl)Cl.CO>COc1cc2c(cc1OC1(C(=O)O)C=CC=CN1)nc(Nc1ccc(Cl)cc1)n2C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-25969f1c4fc64f5496562ec0d510d29a
COc1cc2c(cc1OC1(C(=O)O)C=CC=CN1)nc(Nc1ccc(Cl)cc1)n2C.NCCN1CCCC1>>COc1cc2c(cc1Oc1ccnc(C(=O)NCCN3CCCC3)c1)nc(Nc1ccc(Cl)cc1)n2C
ClC1=CC=C(C=C1)NC1=NC2=C(N1C)C=C(C(=C2)OC2(NC=CC=C2)C(=O)O)OC.N1(CCCC1)CCN.CN(C)C(=[N+](C)C)ON1C2=C(C=CC=C2)N=N1.F[P-](F)(F)(F)(F)F.C(C)(C)N(C(C)C)CC>>ClC1=CC=C(C=C1)NC1=NC2=C(N1C)C=C(C(=C2)OC2=CC(=NC=C2)C(=O)NCCN2CCCC2)OC
O[C:15]([C:10]1([O:9][c:8]2[c:3]([O:2][CH3:1])[cH:4][c:5]3[c:6]([cH:7]2)[n:26][c:27]([NH:28][c:29]2[cH:30][cH:31][c:32]([Cl:33])[cH:34][cH:35]2)[n:36]3[CH3:37])[NH:13][CH:12]=[CH:11][CH:14]=[CH:25]1)=[O:16].[NH2:17][CH2:18][CH2:19][N:20]1[CH2:21][CH2:22][CH2:23][CH2:24]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([cH:7][c:8]...
COc1cc2c(cc1OC1(C(=O)O)C=CC=CN1)nc(Nc1ccc(Cl)cc1)n2C.NCCN1CCCC1
COc1cc2c(cc1Oc1ccnc(C(=O)NCCN3CCCC3)c1)nc(Nc1ccc(Cl)cc1)n2C
null
null
O1CCCC1
Aromatic Heterocycle Formation
OtherReaction
94a4caa66bccd8e91e7b580a9f4a3c5157ecfe3b07bd32b3f62ac4bbe934c768
41c50182f03618bf5d6f37d7b2d64e215c63c1f5eafd63156eb9376a8393c769
O=C(NCCN1CCCC1)c1cc(Oc2ccc3[nH]c(Nc4ccccc4)nc3c2)ccn1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C;H0;D4;+0:3]1(-[#8:4]-[c:5])-[CH;D2;+0:6]=[CH;D2;+0:7]-[CH;D2;+0:8]=[CH;D2;+0:9]-[NH;D2;+0:10]-1.[C:11]-[C:12]-[NH2;D1;+0:13]>>[C:11]-[C:12]-[NH;D2;+0:13]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c;H0;D3;+0:7]1:[cH;D2;+0:6]:[c;H0;D3;+0:3](-[#8:4]-[c:5]):[cH;D2;+0:8]:[cH;D2;+0:9]:[n;H0;D2;+0:10]:1
null
[]
null
null
16
HOUR
To 4-(2-{[4-chloropheylamino)-6-methoxy-1-methylbenzimidazol-5-yloxy)-pyridine-2-carboxylic acid(1 eq) in tetrahydrofuran was added 2-pyrrolidinylethylamine (2 eq), HBTU (2 eq) and N,N-diisopropylethylamine (4 eq) and stir at ambient temperature for 16 h. The mixture was then concentrated and partitioned between ethyl ...
10.6084/m9.figshare.5104873.v1
null
Enamine.Carboxylic acid.Ether.Primary amine.Conjugated diene
Ether.Secondary amide
C1=CCNC=C1
c1ccncc1
c1ccncc1.C1CC[NH]C1.c1ccc2[nH]cnc2c1.c1ccccc1
HO-
O1CCCC1
null
16
COc1cc2c(cc1OC1(C(=O)O)C=CC=CN1)nc(Nc1ccc(Cl)cc1)n2C.NCCN1CCCC1>O1CCCC1>COc1cc2c(cc1Oc1ccnc(C(=O)NCCN3CCCC3)c1)nc(Nc1ccc(Cl)cc1)n2C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-fafcfcb36bd240f0b0d7485f30e31c96
CNc1cc(OC)c(Oc2ccnc(C(=O)OC(C)(C)C)c2)cc1N.Cc1cc(Nc2nc3cc(Oc4ccnc(C(=O)OC(C)(C)C)c4)ccc3n2C)ccc1Br>>COc1cc2c(cc1OC1(C(=O)O)C=CC=CN1)nc(Nc1ccc(Br)c(C)c1)n2C
C(C)(C)(C)OC(=O)C1=NC=CC(=C1)OC1=CC2=C(N(C(=N2)NC2=CC(=C(C=C2)Br)C)C)C=C1.C(C)(C)(C)OC(=O)C1=NC=CC(=C1)OC1=CC(=C(C=C1OC)NC)N.NC(=S)N.FC(C(=O)O)(F)F.IC>>BrC1=C(C=C(C=C1)NC1=NC2=C(N1C)C=C(C(=C2)OC2(NC=CC=C2)C(=O)O)OC)C
CNc1c(N)[cH:7][c:8]([O:9][c:10]2[cH:14][c:15]([C:11](=[O:12])[O:13]C(C)(C)C)[n:18][cH:17][cH:16]2)[c:3]([O:2][CH3:1])[cH:4]1.CC(C)(C)OC(=O)c1cc(Oc2cc[c:5]3[c:6](c2)[n:19][c:20]([NH:21][c:22]2[cH:23][cH:24][c:25]([Br:26])[c:27]([CH3:28])[cH:29]2)[n:30]3[CH3:31])ccn1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([cH:7][c:8]1[O:9]...
CNc1cc(OC)c(Oc2ccnc(C(=O)OC(C)(C)C)c2)cc1N.Cc1cc(Nc2nc3cc(Oc4ccnc(C(=O)OC(C)(C)C)c4)ccc3n2C)ccc1Br
COc1cc2c(cc1OC1(C(=O)O)C=CC=CN1)nc(Nc1ccc(Br)c(C)c1)n2C
null
null
C(Cl)Cl.CO
C-C Coupling
OtherReaction
29efb81d47594bacad1863038bfbc6613a20e196cacf2349980ec228b88f5977
4edbc5aa10c177b20f61383c702da22155b87866fa39db7fef23ed8b6baa10fc
C1=CNC(Oc2ccc3[nH]c(Nc4ccccc4)nc3c2)C=C1
C-C(-C)(-C)-O-C(=O)-c1:c:c(-O-c2:c:c:[c;H0;D3;+0:1]3:[#7;a:2](-[C;D1;H3:3]):[c:4](-[#7:5]):[#7;a:6]:[c;H0;D3;+0:7]:3:c:2):c:c:n:1.C-N-c1:[cH;D2;+0:8]:[c:9](-[#8:10]):[c:11](-[#8:12]-[c;H0;D3;+0:13]2:[cH;D2;+0:14]:[c;H0;D3;+0:15](-[C;H0;D3;+0:16](=[O;D1;H0:17])-[O;H0;D2;+0:18]-C(-C)(-C)-C):[n;H0;D2;+0:19]:[cH;D2;+0:20]:...
null
[]
null
null
16
HOUR
To tert-butyl4-[3-amino-6-methoxy-4-(methylamino)phenoxy]pyridine-2-carboxylate(1 eq) in methanol was added 4-bromo-3-methylbenzeneisothiocyanate (1 eq) and stir at ambient temperature for 16 h. Formation of the corresponding thiourea was followed by LC/MS. To it was then added iodomethane (1 eq) and heated to 60° C. f...
10.6084/m9.figshare.5104873.v1
null
Ester.Ester.Ether.Ether.Primary amine.Secondary amine.Boc.Boc
Enamine.Carboxylic acid.Ether.Conjugated diene
c1ccccc1.c1ccncc1.c1ccncc1.c1nc2ccccc2[nH]1
C1=CCNC=C1.c1ccc2[nH]cnc2c1
C1=CCNC=C1.c1ccc2[nH]cnc2c1.c1ccccc1
HO-
C(Cl)Cl.CO
null
16
CNc1cc(OC)c(Oc2ccnc(C(=O)OC(C)(C)C)c2)cc1N.Cc1cc(Nc2nc3cc(Oc4ccnc(C(=O)OC(C)(C)C)c4)ccc3n2C)ccc1Br>C(Cl)Cl.CO>COc1cc2c(cc1OC1(C(=O)O)C=CC=CN1)nc(Nc1ccc(Br)c(C)c1)n2C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-6577e9885f96489091e1c86056a89b32
COc1cc2c(cc1OC1(C(=O)O)C=CC=CN1)nc(Nc1ccc(Br)c(C)c1)n2C.NCCN1CCCC1>>COc1cc2c(cc1Oc1ccnc(C(=O)NCCN3CCCC3)c1)nc(Nc1ccc(Br)c(C)c1)n2C
BrC1=C(C=C(C=C1)NC1=NC2=C(N1C)C=C(C(=C2)OC2(NC=CC=C2)C(=O)O)OC)C.N1(CCCC1)CCN.CN(C)C(=[N+](C)C)ON1C2=C(C=CC=C2)N=N1.F[P-](F)(F)(F)(F)F.C(C)(C)N(C(C)C)CC>>BrC1=C(C=C(C=C1)NC1=NC2=C(N1C)C=C(C(=C2)OC2=CC(=NC=C2)C(=O)NCCN2CCCC2)OC)C
O[C:15]([C:10]1([O:9][c:8]2[c:3]([O:2][CH3:1])[cH:4][c:5]3[c:6]([cH:7]2)[n:26][c:27]([NH:28][c:29]2[cH:30][cH:31][c:32]([Br:33])[c:34]([CH3:35])[cH:36]2)[n:37]3[CH3:38])[NH:13][CH:12]=[CH:11][CH:14]=[CH:25]1)=[O:16].[NH2:17][CH2:18][CH2:19][N:20]1[CH2:21][CH2:22][CH2:23][CH2:24]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([c...
COc1cc2c(cc1OC1(C(=O)O)C=CC=CN1)nc(Nc1ccc(Br)c(C)c1)n2C.NCCN1CCCC1
COc1cc2c(cc1Oc1ccnc(C(=O)NCCN3CCCC3)c1)nc(Nc1ccc(Br)c(C)c1)n2C
null
null
O1CCCC1
Aromatic Heterocycle Formation
OtherReaction
94a4caa66bccd8e91e7b580a9f4a3c5157ecfe3b07bd32b3f62ac4bbe934c768
41c50182f03618bf5d6f37d7b2d64e215c63c1f5eafd63156eb9376a8393c769
O=C(NCCN1CCCC1)c1cc(Oc2ccc3[nH]c(Nc4ccccc4)nc3c2)ccn1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C;H0;D4;+0:3]1(-[#8:4]-[c:5])-[CH;D2;+0:6]=[CH;D2;+0:7]-[CH;D2;+0:8]=[CH;D2;+0:9]-[NH;D2;+0:10]-1.[C:11]-[C:12]-[NH2;D1;+0:13]>>[C:11]-[C:12]-[NH;D2;+0:13]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c;H0;D3;+0:7]1:[cH;D2;+0:6]:[c;H0;D3;+0:3](-[#8:4]-[c:5]):[cH;D2;+0:8]:[cH;D2;+0:9]:[n;H0;D2;+0:10]:1
null
[]
null
null
16
HOUR
To 4-(2-{[4-bromo-3-methylpheylamino)-6-methoxy-1-methylbenzimidazol-5-yloxy)pyridine-2-carboxylic acid(1 eq) in tetrahydrofuran was added 2-pyrrolidinylethylamine (2 eq), HBTU (2 eq) and N,N-diisopropylethylamine (4 eq) and stir at ambient temperature for 16 h. The mixture was then concentrated and partitioned between...
10.6084/m9.figshare.5104873.v1
null
Enamine.Carboxylic acid.Ether.Primary amine.Conjugated diene
Ether.Secondary amide
C1=CCNC=C1
c1ccncc1
c1ccncc1.C1CC[NH]C1.c1ccc2[nH]cnc2c1.c1ccccc1
HO-
O1CCCC1
null
16
COc1cc2c(cc1OC1(C(=O)O)C=CC=CN1)nc(Nc1ccc(Br)c(C)c1)n2C.NCCN1CCCC1>O1CCCC1>COc1cc2c(cc1Oc1ccnc(C(=O)NCCN3CCCC3)c1)nc(Nc1ccc(Br)c(C)c1)n2C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-7dfe9877116b4fdba75da3ae47db6221
Cc1ccc([N+](=O)[O-])cc1Br.OB(O)c1ccncc1Cl>>Cc1ccc([N+](=O)[O-])cc1-c1ccncc1Cl
BrC1=C(C=CC(=C1)[N+](=O)[O-])C.O.ClC=1C=NC=CC1B(O)O.C([O-])([O-])=O.[Na+].[Na+]>>ClC=1C=NC=CC1C1=C(C=CC(=C1)[N+](=O)[O-])C
Br[c:10]1[c:2]([CH3:1])[cH:3][cH:4][c:5]([N+:6](=[O:7])[O-:8])[cH:9]1.OB(O)[c:11]1[cH:12][cH:13][n:14][cH:15][c:16]1[Cl:17]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([N+:6](=[O:7])[O-:8])[cH:9][c:10]1-[c:11]1[cH:12][cH:13][n:14][cH:15][c:16]1[Cl:17]
Cc1ccc([N+](=O)[O-])cc1Br.OB(O)c1ccncc1Cl
Cc1ccc([N+](=O)[O-])cc1-c1ccncc1Cl
null
[Pd](Cl)Cl.C1(=CC=CC=C1)P(C1=CC=CC=C1)[C-]1C=CC=C1.[C-]1(C=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.[Fe+2]
O.C(OC)COC
C-C Coupling
Suzuki coupling with boronic acids
07e9b6e71d806aa92d4573f3838e77c7c8344de3e5d5735ebdb5fc6862ebf27d
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccncc2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[C;D1;H3:5]):[c:6].O-B(-O)-[c;H0;D3;+0:7]1:[c:8]:[c:9]:[#7;a:10]:[c:11]:[c:12]:1-[Cl;D1;H0:13]>>[C;D1;H3:5]-[c:4](:[c:6]):[c;H0;D3;+0:1](-[c;H0;D3;+0:7]1:[c:8]:[c:9]:[#7;a:10]:[c:11]:[c:12]:1-[Cl;D1;H0:13]):[c:2]:[c:3]
null
[]
90
CELSIUS
null
null
Nitrogen was bubbled through a solution of 2-bromo-1-methyl-4-nitrobenzene (1 eq) in dimethoxyethane and water (3:1) for 0.5 h. Bis(diphenylphosphino)ferrocene Palladium(II)chloride (0.05 eq) followed by 3-chloro-4-pyridine boronic acid hydrate (1 eq) and sodium carbonate (3 eq) was added and the mixture was heated to ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccncc1
c1ccccc1.c1ccncc1
c1ccccc1.c1ccncc1
HBr.B
[Pd](Cl)Cl.C1(=CC=CC=C1)P(C1=CC=CC=C1)[C-]1C=CC=C1.[C-]1(C=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.[Fe+2].O.C(OC)COC
90
null
Cc1ccc([N+](=O)[O-])cc1Br.OB(O)c1ccncc1Cl>[Pd](Cl)Cl.C1(=CC=CC=C1)P(C1=CC=CC=C1)[C-]1C=CC=C1.[C-]1(C=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.[Fe+2].O.C(OC)COC>Cc1ccc([N+](=O)[O-])cc1-c1ccncc1Cl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a524bdbd092c48ae93d277d963df4803
Cc1ccc([N+](=O)[O-])cc1-c1ccncc1Cl>>Cc1ccc(N)cc1-c1ccncc1Cl
ClC=1C=NC=CC1C1=C(C=CC(=C1)[N+](=O)[O-])C.C([O-])([O-])=O.[Na+].[Na+]>>ClC=1C=NC=CC1C=1C=C(C=CC1C)N
O=[N+:6]([O-])[c:5]1[cH:4][cH:3][c:2]([CH3:1])[c:8](-[c:9]2[cH:10][cH:11][n:12][cH:13][c:14]2[Cl:15])[cH:7]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([NH2:6])[cH:7][c:8]1-[c:9]1[cH:10][cH:11][n:12][cH:13][c:14]1[Cl:15]
Cc1ccc([N+](=O)[O-])cc1-c1ccncc1Cl
Cc1ccc(N)cc1-c1ccncc1Cl
null
[Fe]
C(C)(=O)O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc(-c2ccncc2)cc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
6
HOUR
To the mixture containing 3-chloro-4-(2-methyl-5-nitrophenyl)pyridine in acetic acid was added Fe dust (5 eq) and the resulting mixture was stirred at ambient temperature for 6 h. To it was then added saturated sodium carbonate to bring it to neutral pH and extracted with ethyl acetate. The organic layer was washed wit...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1.c1ccncc1
Other
[Fe].C(C)(=O)O
null
6
Cc1ccc([N+](=O)[O-])cc1-c1ccncc1Cl>[Fe].C(C)(=O)O>Cc1ccc(N)cc1-c1ccncc1Cl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-47ebf50a5cb54e36b6b88c98a9f9c59c
CNC(=O)c1cccc(Cl)c1.CNc1cc(OC)c(O)cc1[N+](=O)[O-]>>CNC(=O)c1cc(Oc2cc([N+](=O)[O-])c(NC)cc2OC)ccn1
ClC=1C=C(C=CC1)C(=O)NC.C([O-])([O-])=O.[K+].[K+].COC1=C(C=C(C(=C1)NC)[N+](=O)[O-])O.CC(C)([O-])C.[K+].CN(C(C)=O)C>>COC1=C(OC2=CC(=NC=C2)C(=O)NC)C=C(C(=C1)NC)[N+](=O)[O-]
Cl[c:7]1[cH:6][c:5]([C:3]([NH:2][CH3:1])=[O:4])c[cH:23][cH:22]1.[OH:8][c:9]1[cH:10][c:11]([N+:12](=[O:13])[O-:14])[c:15]([NH:16][CH3:17])[cH:18][c:19]1[O:20][CH3:21]>>[CH3:1][NH:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([O:8][c:9]2[cH:10][c:11]([N+:12](=[O:13])[O-:14])[c:15]([NH:16][CH3:17])[cH:18][c:19]2[O:20][CH3:21])[cH:22][...
CNC(=O)c1cccc(Cl)c1.CNc1cc(OC)c(O)cc1[N+](=O)[O-]
CNC(=O)c1cc(Oc2cc([N+](=O)[O-])c(NC)cc2OC)ccn1
null
null
null
Protection
OtherReaction
f0023f5cb78e4f43639596fb9d7e792c21b5d63a2c4e24a596c544a93eb8f3cf
cf1075be1c1ecf3bb8058899ddc12870a38487ecc9322d6e66205e53a46d9b16
c1ccc(Oc2ccncc2)cc1
Cl-[c;H0;D3;+0:1]1:[c:2]:[cH;D2;+0:3]:c:[c;H0;D3;+0:4](-[C:5](=[O;D1;H0:6])-[#7:7]-[C;D1;H3:8]):[c:9]:1.[OH;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[C;D1;H3:8]-[#7:7]-[C:5](=[O;D1;H0:6])-[c;H0;D3;+0:4]1:[#7;a:14]:[cH;D2;+0:3]:[c:2]:[c;H0;D3;+0:1](-[O;H0;D2;+0:10]-[c:11](:[c:12]):[c:13]):[c:9]:1
null
[]
null
null
null
null
To a stirred solution of 2-methoxy-4-(methylamino)-5-nitrophenol(1 eq) in N,N-dimethylacetamide was added potassium-t-butoxide (1.2 eq) and continued stirring at ambient temperature until it solidified. To it was then added (3-chlorophenyl)-N-methylcarboxamide (1 eq) and anhydrous potassium carbonate (1 eq) and the res...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccccc1
c1ccncc1
c1ccncc1.c1ccccc1
HCl
null
null
null
CNC(=O)c1cccc(Cl)c1.CNc1cc(OC)c(O)cc1[N+](=O)[O-]>>CNC(=O)c1cc(Oc2cc([N+](=O)[O-])c(NC)cc2OC)ccn1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ece00de1a8ae45ebb41ea31a86d1e23b
CNC(=O)c1cc(Oc2cc([N+](=O)[O-])c(NC)cc2OC)ccn1>>CNC(=O)c1cc(Oc2cc(N)c(NC)cc2OC)ccn1
COC1=C(OC2=CC(=NC=C2)C(=O)NC)C=C(C(=C1)NC)[N+](=O)[O-]>>NC=1C=C(OC2=CC(=NC=C2)C(=O)NC)C(=CC1NC)OC
O=[N+:12]([O-])[c:11]1[cH:10][c:9]([O:8][c:7]2[cH:6][c:5]([C:3]([NH:2][CH3:1])=[O:4])[n:22][cH:21][cH:20]2)[c:17]([O:18][CH3:19])[cH:16][c:13]1[NH:14][CH3:15]>>[CH3:1][NH:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([O:8][c:9]2[cH:10][c:11]([NH2:12])[c:13]([NH:14][CH3:15])[cH:16][c:17]2[O:18][CH3:19])[cH:20][cH:21][n:22]1
CNC(=O)c1cc(Oc2cc([N+](=O)[O-])c(NC)cc2OC)ccn1
CNC(=O)c1cc(Oc2cc(N)c(NC)cc2OC)ccn1
null
[Pd]
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc(Oc2ccncc2)cc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
A solution of {4-[2-methoxy-4-(methylamino)-5-nitrophenoxy](2-pyridyl)}-N-methylcarboxamide. In methanol was hydrogenated with 10% Pd/C. The catalyst was filtered off and the solvent was concentrated to yield {4-[3-amino-6-methoxy-4-(methylamino)phenoxy](2-pyridyl)}-N-methylcarboxamide. MS :MH+: 302. Conditions: See re...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccncc1.c1ccccc1
Other
[Pd].CO
null
null
CNC(=O)c1cc(Oc2cc([N+](=O)[O-])c(NC)cc2OC)ccn1>[Pd].CO>CNC(=O)c1cc(Oc2cc(N)c(NC)cc2OC)ccn1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f7c91842ad414fc4bf824d4efcc8346b
COC(=O)c1cncc(Oc2ccc([N+](=O)[O-])cc2)c1>>COC(=O)c1cncc(Oc2ccc(N)cc2)c1
COC(=O)C=1C=NC=C(C1)OC1=CC=C(C=C1)[N+](=O)[O-]>>COC(=O)C=1C=NC=C(C1)OC1=CC=C(C=C1)N
O=[N+:15]([O-])[c:14]1[cH:13][cH:12][c:11]([O:10][c:9]2[cH:8][n:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:18]2)[cH:17][cH:16]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][n:7][cH:8][c:9]([O:10][c:11]2[cH:12][cH:13][c:14]([NH2:15])[cH:16][cH:17]2)[cH:18]1
COC(=O)c1cncc(Oc2ccc([N+](=O)[O-])cc2)c1
COC(=O)c1cncc(Oc2ccc(N)cc2)c1
null
[Pd]
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc(Oc2cccnc2)cc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
The mixture containing methyl-5-(4-nitrophenoxy)pyridine-3-carboxylate in methanol with catalytic amount of 10% Pd/C was hydrogenated to yield methyl5-[4-aminophenoxy]pyridine-3-carboxylate. MS: MH+=244. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccncc1.c1ccccc1
Other
[Pd].CO
null
null
COC(=O)c1cncc(Oc2ccc([N+](=O)[O-])cc2)c1>[Pd].CO>COC(=O)c1cncc(Oc2ccc(N)cc2)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-bb9a850ef83945038bd3835d81d78414
COC(=O)c1cncc(Oc2ccc(NC(=O)C(F)(F)F)c([N+](=O)[O-])c2)c1.COS(=O)(=O)OC>>CNc1ccc(Oc2ccncc2C(=O)OC)cc1[N+](=O)[O-]
S(=O)(=O)(OC)OC.COC(=O)C=1C=NC=C(C1)OC1=CC(=C(C=C1)NC(C(F)(F)F)=O)[N+](=O)[O-].C(C)#N.[OH-].[Na+].C1(=CC=CC=C1)C>>COC(=O)C=1C=NC=CC1OC1=CC(=C(C=C1)NC)[N+](=O)[O-]
O=C(C(F)(F)F)[NH:2][c:3]1[cH:4][cH:5][c:6]([O:7][c:8]2[cH:9][c:13]([C:14](=[O:15])[O:16][CH3:17])[cH:12][n:11][cH:10]2)[cH:18][c:19]1[N+:20](=[O:21])[O-:22].COS(=O)(=O)O[CH3:1]>>[CH3:1][NH:2][c:3]1[cH:4][cH:5][c:6]([O:7][c:8]2[cH:9][cH:10][n:11][cH:12][c:13]2[C:14](=[O:15])[O:16][CH3:17])[cH:18][c:19]1[N+:20](=[O:21])[...
COC(=O)c1cncc(Oc2ccc(NC(=O)C(F)(F)F)c([N+](=O)[O-])c2)c1.COS(=O)(=O)OC
CNc1ccc(Oc2ccncc2C(=O)OC)cc1[N+](=O)[O-]
null
[Cl-].C(C1=CC=CC=C1)[N+](C)(C)C
null
Functional Group Addition
OtherReaction
4e8b58513939f305220516ba66a29c403383c4fdcb5862eba3a3a67db4b3baff
d1cd17b8c44f4dd4dd342fb29e5927608ceb97f81a8ca71bbe503b983f1461f9
c1ccc(Oc2ccncc2)cc1
C-O-S(=O)(=O)-O-[CH3;D1;+0:1].F-C(-F)(-F)-C(=O)-[NH;D2;+0:2]-[c:3](:[c:4]):[c:5].[C;D1;H3:6]-[#8:7]-[C:8](=[O;D1;H0:9])-[c;H0;D3;+0:10]1:[c:11]:[#7;a:12]:[cH;D2;+0:13]:[c;H0;D3;+0:14](-[#8:15]-[c:16]):[cH;D2;+0:17]:1>>[C;D1;H3:6]-[#8:7]-[C:8](=[O;D1;H0:9])-[c;H0;D3;+0:10]1:[c:11]:[#7;a:12]:[cH;D2;+0:13]:[cH;D2;+0:17]:[...
null
[]
null
null
8
HOUR
To the solution of the methyl5-[3-nitro-4-(2,2,2-trifluroacetylamino)phenoxy]-pyridine-3-carboxylate (1 eq) in a mixture of toluene, acetonitrile and sodium hydroxide solution (50%) was added benzyltrimethylammonium chloride (1 eq) and dimethyl sulfate (1.2 eq). The biphasic mixture was stirred overnight at room temper...
10.6084/m9.figshare.5104873.v1
null
Trifluoro group.Ester.Ether.Secondary amide
Ester.Ether.Secondary amine
c1ccncc1
c1ccncc1
c1ccccc1.c1ccncc1
HF
[Cl-].C(C1=CC=CC=C1)[N+](C)(C)C
null
8
COC(=O)c1cncc(Oc2ccc(NC(=O)C(F)(F)F)c([N+](=O)[O-])c2)c1.COS(=O)(=O)OC>[Cl-].C(C1=CC=CC=C1)[N+](C)(C)C>CNc1ccc(Oc2ccncc2C(=O)OC)cc1[N+](=O)[O-]
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f88b00a854de4ae3bb737e32aeb6ea63
CNc1ccc(Oc2cncc(C(=O)OC)c2)cc1N.S=C=Nc1ccc(Br)cc1>>COC(=O)c1cncc(Oc2ccc3c(c2)nc(Nc2ccc(Br)cc2)n3C)c1
CI.COC(=O)C=1C=NC=C(C1)OC1=CC(=C(C=C1)NC)N.BrC1=CC=C(C=C1)N=C=S>>COC(=O)C=1C=NC=C(C1)OC1=CC2=C(N(C(=N2)NC2=CC=C(C=C2)Br)C)C=C1
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][n:7][cH:8][c:9]([O:10][c:11]2[cH:12][cH:13][c:14]([NH:27][CH3:28])[c:15]([NH2:17])[cH:16]2)[cH:29]1.S=[C:18]=[N:19][c:20]1[cH:21][cH:22][c:23]([Br:24])[cH:25][cH:26]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][n:7][cH:8][c:9]([O:10][c:11]2[cH:12][cH:13][c:14]3[c:15]([cH:16]2)[n:17][c:1...
CNc1ccc(Oc2cncc(C(=O)OC)c2)cc1N.S=C=Nc1ccc(Br)cc1
COC(=O)c1cncc(Oc2ccc3c(c2)nc(Nc2ccc(Br)cc2)n3C)c1
null
null
CO
Aromatic Heterocycle Formation
OtherReaction
d7416f6ffd0cf3a591ff39bb82719e0121b02095a886f4bf34a4bce30d165f53
c2745d0d96944794048cb0a435469fb3c0efa689f6d5e8d4fd6447372cabc5f8
c1ccc(Nc2nc3cc(Oc4cccnc4)ccc3[nH]2)cc1
S=[C;H0;D2;+0:1]=[N;H0;D2;+0:2]-[c:3](:[c:4]):[c:5].[C;D1;H3:6]-[NH;D2;+0:7]-[c:8](:[c:9]):[c:10](-[NH2;D1;+0:11]):[c:12]>>[C;D1;H3:6]-[n;H0;D3;+0:7]1:[c:8](:[c:9]):[c:10](:[c:12]):[n;H0;D2;+0:11]:[c;H0;D3;+0:1]:1-[NH;D2;+0:2]-[c:3](:[c:4]):[c:5]
null
[]
null
null
2
HOUR
A solution of the methyl5-[3-amino-4-(methylamino)phenoxy]pyridine-3-carboxylate (1 eq) in methanol (8 ml) was treated with 4-bromophenylisothiocyanate (1 eq) and stirred at 60° C.–65° C. for 2 hours. The reaction mixture was cooled down to room temperature and methyl iodide (1 eq) was added and stirred overnight at 60...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Secondary amine.Isothiocyanate
Secondary amine
c1ccccc1
c1ccc2nc[nH]c2c1
c1ccncc1.c1ccc2nc[nH]c2c1.c1ccccc1
Other
CO
null
2
CNc1ccc(Oc2cncc(C(=O)OC)c2)cc1N.S=C=Nc1ccc(Br)cc1>CO>COC(=O)c1cncc(Oc2ccc3c(c2)nc(Nc2ccc(Br)cc2)n3C)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-3c5e0b6c49554f4aae13c05d3f715346
CN.COC(=O)c1cncc(Oc2ccc3c(c2)nc(Nc2ccc(Br)cc2)n3C)c1>>CNC(=O)c1cncc(Oc2ccc3c(c2)nc(Nc2ccc(Br)cc2)n3C)c1
COC(=O)C=1C=NC=C(C1)OC1=CC2=C(N(C(=N2)NC2=CC=C(C=C2)Br)C)C=C1.CN>>BrC1=CC=C(C=C1)NC1=NC2=C(N1C)C=CC(=C2)OC=2C=C(C=NC2)C(=O)NC
[CH3:1][NH2:2].CO[C:3](=[O:4])[c:5]1[cH:6][n:7][cH:8][c:9]([O:10][c:11]2[cH:12][cH:13][c:14]3[c:15]([cH:16]2)[n:17][c:18]([NH:19][c:20]2[cH:21][cH:22][c:23]([Br:24])[cH:25][cH:26]2)[n:27]3[CH3:28])[cH:29]1>>[CH3:1][NH:2][C:3](=[O:4])[c:5]1[cH:6][n:7][cH:8][c:9]([O:10][c:11]2[cH:12][cH:13][c:14]3[c:15]([cH:16]2)[n:17][c...
CN.COC(=O)c1cncc(Oc2ccc3c(c2)nc(Nc2ccc(Br)cc2)n3C)c1
CNC(=O)c1cncc(Oc2ccc3c(c2)nc(Nc2ccc(Br)cc2)n3C)c1
null
null
null
Acylation
Aminolysis of esters
04c54ce22aa9bc0cea0de3d900446bcab51cf02bebeb606fa788a47dcd0e37ff
4335147c9ad02004b7c12428d7eac0b2e7e0e2017adc471d01c387239de8017d
c1ccc(Nc2nc3cc(Oc4cccnc4)ccc3[nH]2)cc1
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]:[#7;a:6]:[c:7].[C;D1;H3:8]-[NH2;D1;+0:9]>>[C;D1;H3:8]-[NH;D2;+0:9]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]:[#7;a:6]:[c:7]
null
[]
null
null
null
null
To a solution of methyl5-{2-[(4-bromophenyl)amino]-1-methylbenzimidazol-5-yloxy}pyridine-3-carboxylate in added methylamine and the resulting mixture was stirred at ambient temperature for 16 h. It was then concentrated and purified by preparative chromatography to yield (5-{2-[(4-bromophenyl)amino]-1-methylbenzimidazo...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine
Secondary amide
null
null
c1ccncc1.c1ccc2nc[nH]c2c1.c1ccccc1
HO-
null
null
null
CN.COC(=O)c1cncc(Oc2ccc3c(c2)nc(Nc2ccc(Br)cc2)n3C)c1>>CNC(=O)c1cncc(Oc2ccc3c(c2)nc(Nc2ccc(Br)cc2)n3C)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0d4cc39a59824b21916c9f11a96a886e
CNC.O=[N+]([O-])c1ccc(Cl)nc1>>CN(C)c1ccc([N+](=O)[O-])cn1
ClC1=NC=C(C=C1)[N+](=O)[O-].CNC.O>>CN(C1=NC=C(C=C1)[N+](=O)[O-])C
[CH3:1][NH:2][CH3:3].Cl[c:4]1[cH:5][cH:6][c:7]([N+:8](=[O:9])[O-:10])[cH:11][n:12]1>>[CH3:1][N:2]([CH3:3])[c:4]1[cH:5][cH:6][c:7]([N+:8](=[O:9])[O-:10])[cH:11][n:12]1
CNC.O=[N+]([O-])c1ccc(Cl)nc1
CN(C)c1ccc([N+](=O)[O-])cn1
null
null
CN1CCCC1=O
Heteroatom Alkylation and Arylation
Ullmann-Goldberg Substitution amine
a0163952e7575991d15970b416e74bb56cf346e5420a42d8fb74b35140502d0d
b6b8e2cdb45054a35f5e8157d624f852c0601a09401556706e166b19536eb7a7
c1ccncc1
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5].[C;D1;H3:6]-[NH;D2;+0:7]-[C;D1;H3:8]>>[C;D1;H3:6]-[N;H0;D3;+0:7](-[C;D1;H3:8])-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4]:[c:5]
null
[]
null
null
null
null
2-Chloro-5-nitropyridine (1.0 eq) and dimethylamine (2 M in EtOH, 4.6 eq) in NMP were heated for 2 h at 100° C. The solution was then poured slowly into H2O. The filtrate that formed was filtered and dried to give 2-(dimethylamino)-5-nitropyridine. Conditions: See reaction.notes.procedure_details. Workup: The filtrate ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Secondary amine
Tertiary amine
c1ccncc1
c1ccncc1
c1ccncc1
HCl
CN1CCCC1=O
null
null
CNC.O=[N+]([O-])c1ccc(Cl)nc1>CN1CCCC1=O>CN(C)c1ccc([N+](=O)[O-])cn1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-646ee376cd9a44aaa4321c391e2fa201
CN(C)c1ccc([N+](=O)[O-])cn1>>CN(C)c1ccc(N)cn1
CN(C1=NC=C(C=C1)[N+](=O)[O-])C>>CN(C1=NC=C(C=C1)N)C
O=[N+:8]([O-])[c:7]1[cH:6][cH:5][c:4]([N:2]([CH3:1])[CH3:3])[n:10][cH:9]1>>[CH3:1][N:2]([CH3:3])[c:4]1[cH:5][cH:6][c:7]([NH2:8])[cH:9][n:10]1
CN(C)c1ccc([N+](=O)[O-])cn1
CN(C)c1ccc(N)cn1
null
[Pd]
C(C)O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccncc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]:[#7;a:5]:[c:6]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]:[#7;a:5]:[c:6]
null
[]
null
null
8
HOUR
A mixture of 2-(dimethylamino)-5-nitropyridine (1 eq) and 5% palladium on carbon (0.3 eq) in ethanol was stirred at room temperature and flushed with nitrogen. The reaction vessel was evacuated and purged with hydrogen three times. The reaction mixture was left under an atmosphere of hydrogen overnight. Nitrogen was fl...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccncc1
Other
[Pd].C(C)O
null
8
CN(C)c1ccc([N+](=O)[O-])cn1>[Pd].C(C)O>CN(C)c1ccc(N)cn1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-8f82121579ef4eca9d6cf6b432beefbd
CNC(=O)c1cc(Oc2ccc(N)c([N+](=O)[O-])c2)ccn1.Nc1ccc(O)cc1[N+](=O)[O-]>>O=[N+]([O-])Nc1ccccc1
C(Cl)Cl.NC1=C(C=C(C=C1)O)[N+](=O)[O-].NC1=C(C=C(OC2=CC(=NC=C2)C(=O)NC)C=C1)[N+](=O)[O-].C([O-])([O-])=O.[Na+].[Na+]>>[N+](=O)([O-])NC1=CC=CC=C1
CNC(=O)c1cc(Oc2ccc(N)c([N+:2](=[O:1])[O-:3])c2)ccn1.O=[N+]([O-])[c:10]1[c:5]([NH2:4])[cH:6][cH:7][c:8](O)[cH:9]1>>[O:1]=[N+:2]([O-:3])[NH:4][c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1
CNC(=O)c1cc(Oc2ccc(N)c([N+](=O)[O-])c2)ccn1.Nc1ccc(O)cc1[N+](=O)[O-]
O=[N+]([O-])Nc1ccccc1
null
null
O.COCCOC.O.C(C)(=O)OCC
Functional Group Addition
OtherReaction
86bc2645c62da628c1b0f146568ee6ae2487f0b469dcadde2d0b02e61a45383c
612c2322ffd5d165f8c3c7313c038638c8ba2e78bb7f92591a7ca3386f36d8f5
c1ccccc1
C-N-C(=O)-c1:c:c(-O-c2:c:c:c(-N):c(-[N+;H0;D3:1](-[O;-;D1;H0:2])=[O;D1;H0:3]):c:2):c:c:n:1.O-[c;H0;D3;+0:4]1:[c:5]:[c:6]:[c:7](-[NH2;D1;+0:8]):[c;H0;D3;+0:9](-[N+](=O)-[O-]):[c:10]:1>>[O;-;D1;H0:2]-[N+;H0;D3:1](=[O;D1;H0:3])-[NH;D2;+0:8]-[c:7]1:[c:6]:[c:5]:[cH;D2;+0:4]:[c:10]:[cH;D2;+0:9]:1
null
[]
100
CELSIUS
null
null
A solution of 5 (1 eq), 6 (1 eq), and sodium carbonate (1.2 eq) in DME/H2O (3:1) was degassed by bubbling argon through the solution for 10 minutes. Pd(II)(dppf)Cl2.MeCl2 (0.1 eq) was added to the reaction solution and the reaction was sealed. The reaction was heated at 100° C. overnight. The reaction was cooled to RT ...
10.6084/m9.figshare.5104873.v1
null
Ether.Nitro group.Nitro group.Secondary amide.Aromatic alcohol.Primary amine.Primary amine
Hydrazine
c1ccncc1.c1ccccc1.c1ccccc1
c1ccccc1
c1ccccc1
HO-
O.COCCOC.O.C(C)(=O)OCC
100
null
CNC(=O)c1cc(Oc2ccc(N)c([N+](=O)[O-])c2)ccn1.Nc1ccc(O)cc1[N+](=O)[O-]>O.COCCOC.O.C(C)(=O)OCC>O=[N+]([O-])Nc1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-33389ec7e72c4df3b9b8deccba4fd745
CC(C)c1cccc(Nc2nc3cc(Oc4ccnc(C(=O)NCCN)c4)ccc3n2C)c1.O=S(=O)(Cl)Cc1ccccc1>>CC(C)c1cccc(Nc2nc3cc(Oc4ccnc(C(=O)NCCNS(=O)(=O)Cc5ccccc5)c4)ccc3n2C)c1
C1(=CC=CC=C1)CS(=O)(=O)Cl.NCCNC(=O)C1=NC=CC(=C1)OC1=CC2=C(N(C(=N2)NC2=CC(=CC=C2)C(C)C)C)C=C1.C(=O)([O-])[O-].[K+].[K+].C(C)#N>>C1(=CC=CC=C1)CS(=O)(=O)NCCNC(=O)C1=NC=CC(=C1)OC1=CC2=C(N(C(=N2)NC2=CC(=CC=C2)C(C)C)C)C=C1
[CH3:1][CH:2]([CH3:3])[c:4]1[cH:5][cH:6][cH:7][c:8]([NH:9][c:10]2[n:11][c:12]3[cH:13][c:14]([O:15][c:16]4[cH:17][cH:18][n:19][c:20]([C:21](=[O:22])[NH:23][CH2:24][CH2:25][NH2:26])[cH:37]4)[cH:38][cH:39][c:40]3[n:41]2[CH3:42])[cH:43]1.Cl[S:27](=[O:28])(=[O:29])[CH2:30][c:31]1[cH:32][cH:33][cH:34][cH:35][cH:36]1>>[CH3:1]...
CC(C)c1cccc(Nc2nc3cc(Oc4ccnc(C(=O)NCCN)c4)ccc3n2C)c1.O=S(=O)(Cl)Cc1ccccc1
CC(C)c1cccc(Nc2nc3cc(Oc4ccnc(C(=O)NCCNS(=O)(=O)Cc5ccccc5)c4)ccc3n2C)c1
null
null
O
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=C(NCCNS(=O)(=O)Cc1ccccc1)c1cc(Oc2ccc3[nH]c(Nc4ccccc4)nc3c2)ccn1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[C:4]-[c:5].[C:6]-[C:7]-[NH2;D1;+0:8]>>[C:6]-[C:7]-[NH;D2;+0:8]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[C:4]-[c:5]
null
[]
null
null
1
HOUR
To a mixture containing 4-[2-(3-Isopropyl-phenylamino)-1-methyl-1H-benzoimidazol-5-yloxy]-pyridine-2-carboxylic acid (2-amino-ethyl)-amide (1 eq) (prepared using previously described example 3), K2CO3 (5 eq), (0.2 M in a 5:1 mixture of acetonitrile and water) were added α-toluenesulfonyl chloride (1 eq) via syringe. Th...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccccc1.c1ccc2nc[nH]c2c1.c1ccncc1.c1ccccc1
HCl
O
null
1
CC(C)c1cccc(Nc2nc3cc(Oc4ccnc(C(=O)NCCN)c4)ccc3n2C)c1.O=S(=O)(Cl)Cc1ccccc1>O>CC(C)c1cccc(Nc2nc3cc(Oc4ccnc(C(=O)NCCNS(=O)(=O)Cc5ccccc5)c4)ccc3n2C)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d83a7c5eff9f4444938f5ef737900e22
CCO.CNC(=O)c1cc(Oc2cc([N+](=O)[O-])c(NC)cc2OC)ccn1>>Nc1ccc(OCCCN2CCCC2)cc1N
COC1=C(OC2=CC(=NC=C2)C(=O)NC)C=C(C(=C1)NC)[N+](=O)[O-].CCO>>N1(CCCC1)CCCOC=1C=C(C(=CC1)N)N
O[CH2:7][CH3:8].C[NH:17][c:16]1[c:2]([N+:1](=O)[O-])[cH:3][c:4]([O:6]c2c[c:9](C(=O)N[CH3:11])[n:10][cH:13][cH:12]2)[c:5](O[CH3:14])[cH:15]1>>[NH2:1][c:2]1[cH:3][cH:4][c:5]([O:6][CH2:7][CH2:8][CH2:9][N:10]2[CH2:11][CH2:12][CH2:13][CH2:14]2)[cH:15][c:16]1[NH2:17]
CCO.CNC(=O)c1cc(Oc2cc([N+](=O)[O-])c(NC)cc2OC)ccn1
Nc1ccc(OCCCN2CCCC2)cc1N
null
[Pd]
null
Functional Group Interconversion
OtherReaction
5c8f9143e2e2766e0dc505bfc1f92c62f37241f237126605047aedf8c18ae9ef
20fd7ea1b0d0bd4bb0c0bb94c83c721be4371db6d08d2db71c2fe642fc3b6a26
c1ccc(OCCCN2CCCC2)cc1
C-[NH;D2;+0:1]-[c:2]1:[c:3]:[c;H0;D3;+0:4](-O-[CH3;D1;+0:5]):[c;H0;D3;+0:6](-[O;H0;D2;+0:7]-c2:[cH;D2;+0:8]:[cH;D2;+0:9]:[n;H0;D2;+0:10]:[c;H0;D3;+0:11](-C(=O)-N-[CH3;D1;+0:12]):c:2):[c:13]:[c:14]:1-[N+;H0;D3:15](=O)-[O-].O-[CH2;D2;+0:16]-[CH3;D1;+0:17]>>[NH2;D1;+0:1]-[c:2]1:[c:3]:[c;H0;D3;+0:4](-[O;H0;D2;+0:7]-[CH2;D2...
null
[]
null
null
18
HOUR
To a solution 2-Nitro-4-(3-pyrrolidinylpropoxy)phenylamine 1 in EtOH, Pd/C (0.1 eq) is added. The reaction vessel is repeatedly purged (×3) with nitrogen, and then stirred under a hydrogen atmosphere for 18 h. The product is filtered through a Celite plug, and the plug washed with 25 mL of EtOH, to yield 2. LCMS 236.2 ...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Nitro group.Secondary amide.Primary alcohol.Secondary amine
Ether.Primary amine.Primary amine.Tertiary amine
c1ccccc1.c1ccncc1
c1ccccc1.C1CC[NH]C1
c1ccccc1.C1CC[NH]C1
HO-
[Pd]
null
18
CCO.CNC(=O)c1cc(Oc2cc([N+](=O)[O-])c(NC)cc2OC)ccn1>[Pd]>Nc1ccc(OCCCN2CCCC2)cc1N
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-93bd734cd93549c9ba3d48b9626f217f
CN1CCNCC1.Nc1cc(F)ccc1[N+](=O)[O-]>>CN1CCN(c2ccc([N+](=O)[O-])c(N)c2)CC1
CN1CCNCC1.CN1CCCC1=O.C(C)N(CC)CC.FC=1C=CC(=C(C1)N)[N+](=O)[O-]>>CN1CCN(CC1)C=1C=CC(=C(C1)N)[N+](=O)[O-]
[CH3:1][N:2]1[CH2:3][CH2:4][NH:5][CH2:16][CH2:17]1.F[c:6]1[cH:7][cH:8][c:9]([N+:10](=[O:11])[O-:12])[c:13]([NH2:14])[cH:15]1>>[CH3:1][N:2]1[CH2:3][CH2:4][N:5]([c:6]2[cH:7][cH:8][c:9]([N+:10](=[O:11])[O-:12])[c:13]([NH2:14])[cH:15]2)[CH2:16][CH2:17]1
CN1CCNCC1.Nc1cc(F)ccc1[N+](=O)[O-]
CN1CCN(c2ccc([N+](=O)[O-])c(N)c2)CC1
null
null
O
Heteroatom Alkylation and Arylation
Buchwald-Hartwig/Ullmann-Goldberg/N-arylation secondary amine
d687b31bdda9f407fdde6ca57e67eee0681e173646c617afef7770c56d05bab9
b6b8e2cdb45054a35f5e8157d624f852c0601a09401556706e166b19536eb7a7
c1ccc(N2CCNCC2)cc1
F-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[#7:6]1-[C:7]-[C:8]-[NH;D2;+0:9]-[C:10]-[C:11]-1>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[N;H0;D3;+0:9]1-[C:8]-[C:7]-[#7:6]-[C:11]-[C:10]-1):[c:4]:[c:5]
null
[]
null
null
12
HOUR
A solution of N-methylpiperazine (1.0 eq), NMP, triethylamine (3.0 eq) and 5-fluoro-2-nitrophenylamine (1.0 eq) were heated at 90° C. for 1 hours. The reaction was allowed to cool to room temperature and then poured into water and let stand for 12 hours. The resulting solid was collected and dried and utilized without ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Secondary amine
Tertiary amine
C1C[NH]CCN1.c1ccccc1
C1C[NH]CC[NH]1.c1ccccc1
C1C[NH]CC[NH]1.c1ccccc1
HF
O
null
12
CN1CCNCC1.Nc1cc(F)ccc1[N+](=O)[O-]>O>CN1CCN(c2ccc([N+](=O)[O-])c(N)c2)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-9dd8ff5a8b8b41219f159bbebd81ad04
CNC(=O)c1cc(Oc2cc([N+](=O)[O-])c(NC)cc2OC)ccn1.S=C=Nc1cccc(Oc2ccccc2)c1>>CNC(=O)c1cc(Oc2ccc3c(c2)nc(Nc2cccc(Oc4ccccc4)c2)n3C)ccn1
O(C1=CC=CC=C1)C=1C=C(C=CC1)N=C=S.COC1=C(OC2=CC(=NC=C2)C(=O)NC)C=C(C(=C1)NC)[N+](=O)[O-].CI>>CNC(=O)C1=NC=CC(=C1)OC1=CC2=C(N(C(=N2)NC2=CC(=CC=C2)OC2=CC=CC=C2)C)C=C1
CO[c:10]1[c:9]([O:8][c:7]2[cH:6][c:5]([C:3]([NH:2][CH3:1])=[O:4])[n:35][cH:34][cH:33]2)[cH:14][c:13]([N+:15](=O)[O-])[c:12]([NH:31][CH3:32])[cH:11]1.S=[C:16]=[N:17][c:18]1[cH:19][cH:20][cH:21][c:22]([O:23][c:24]2[cH:25][cH:26][cH:27][cH:28][cH:29]2)[cH:30]1>>[CH3:1][NH:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([O:8][c:9]2[cH:10...
CNC(=O)c1cc(Oc2cc([N+](=O)[O-])c(NC)cc2OC)ccn1.S=C=Nc1cccc(Oc2ccccc2)c1
CNC(=O)c1cc(Oc2ccc3c(c2)nc(Nc2cccc(Oc4ccccc4)c2)n3C)ccn1
null
null
CO
Aromatic Heterocycle Formation
OtherReaction
e01045c6582f8094924aa12a0ae4155a5e203c3b3b57eaca9716db280dbf92a5
3df5785608eefdb0973d9c896a6050fedd9fdf25c115a747f31ba5969e559ebc
c1ccc(Oc2cccc(Nc3nc4cc(Oc5ccncc5)ccc4[nH]3)c2)cc1
C-O-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[NH;D2;+0:4]-[C;D1;H3:5]):[c:6](-[N+;H0;D3:7](=O)-[O-]):[c:8]:[c:9]:1-[#8:10].S=[C;H0;D2;+0:11]=[N;H0;D2;+0:12]-[c:13](:[c:14]):[c:15]>>[#8:10]-[c:9]1:[c:8]:[c:6]2:[n;H0;D2;+0:7]:[c;H0;D3;+0:11](-[NH;D2;+0:12]-[c:13](:[c:14]):[c:15]):[n;H0;D3;+0:4](-[C;D1;H3:5]):[c:3]:2:[c:2]:[cH;D2;+0:...
null
[]
null
null
8
HOUR
A 1 dram vial was charged with a solution of 3-phenoxyphenylisothiocyanate (23 mg, 0.1 mmol), diamine 1 (27 mg, 0.1 mmol), and MeOH (0.5 mL) and the reaction was shaken at rt overnight. Methyl iodide (8 uL, 0.13 mmol) was added and the mixture shaken overnight. The reaction was concentrated and the resulting residue pu...
10.6084/m9.figshare.5104873.v1
null
Ether.Nitro group.Secondary amine.Isothiocyanate
Secondary amine
c1ccccc1
c1ccc2nc[nH]c2c1
c1ccncc1.c1ccc2nc[nH]c2c1.c1ccccc1.c1ccccc1
Other
CO
null
8
CNC(=O)c1cc(Oc2cc([N+](=O)[O-])c(NC)cc2OC)ccn1.S=C=Nc1cccc(Oc2ccccc2)c1>CO>CNC(=O)c1cc(Oc2ccc3c(c2)nc(Nc2cccc(Oc4ccccc4)c2)n3C)ccn1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-578aafd6133147929ebb566b7654c689
CNC(=O)c1cc(Oc2cc([N+](=O)[O-])c(NC)cc2OC)ccn1.O=Cc1ccc(Br)cc1>>CNC(=O)c1cc(Oc2ccc3c(c2)nc(-c2ccc(Br)cc2)n3C)ccn1
COC1=C(OC2=CC(=NC=C2)C(=O)NC)C=C(C(=C1)NC)[N+](=O)[O-].BrC1=CC=C(C=O)C=C1>>CNC(=O)C1=NC=CC(=C1)OC1=CC2=C(N(C(=N2)C2=CC=C(C=C2)Br)C)C=C1
CO[c:10]1[c:9]([O:8][c:7]2[cH:6][c:5]([C:3]([NH:2][CH3:1])=[O:4])[n:28][cH:27][cH:26]2)[cH:14][c:13]([N+:15](=O)[O-])[c:12]([NH:24][CH3:25])[cH:11]1.O=[CH:16][c:17]1[cH:18][cH:19][c:20]([Br:21])[cH:22][cH:23]1>>[CH3:1][NH:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([O:8][c:9]2[cH:10][cH:11][c:12]3[c:13]([cH:14]2)[n:15][c:16](-[c:...
CNC(=O)c1cc(Oc2cc([N+](=O)[O-])c(NC)cc2OC)ccn1.O=Cc1ccc(Br)cc1
CNC(=O)c1cc(Oc2ccc3c(c2)nc(-c2ccc(Br)cc2)n3C)ccn1
null
null
O1CCOCC1
Aromatic Heterocycle Formation
OtherReaction
e451cfd55755e6b1044f1e94003171c7580983989ef49f333fe1628342897349
106c47f7abe58d817988fc6d996094606a2af5ef5c09dd35fea21b01eadf0288
c1ccc(-c2nc3cc(Oc4ccncc4)ccc3[nH]2)cc1
C-O-[c;H0;D3;+0:1]1:[c:2]:[c:3](-[NH;D2;+0:4]-[C;D1;H3:5]):[c:6](-[N+;H0;D3:7](=O)-[O-]):[c:8]:[c:9]:1-[#8:10].O=[CH;D2;+0:11]-[c;H0;D3;+0:12](:[c:13]:[c:14]):[c:15]:[c:16]>>[#8:10]-[c:9]1:[c:8]:[c:6]2:[n;H0;D2;+0:7]:[c;H0;D3;+0:11](-[c;H0;D3;+0:12](:[c:13]:[c:14]):[c:15]:[c:16]):[n;H0;D3;+0:4](-[C;D1;H3:5]):[c:3]:2:[c...
null
[]
100
CELSIUS
null
null
A mixture of diamine 1 (137 mg, 0.36 mmol) and 4-bromobenzaldehyde (66 mg, 0.50 mmol) in dry dioxane (2 mL) was heated to 100° C. for 16 h. The reaction mixture was allowed to cool to rt and was then concentrated. The resulting residue was purified by reverse phase HPLC to finish 2 as the TFA salt: LCMS m/z 437.1, tR=2...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Ether.Nitro group.Secondary amine
null
c1ccccc1
c1ccc2nc[nH]c2c1
c1ccncc1.c1ccc2nc[nH]c2c1.c1ccccc1
HO-
O1CCOCC1
100
null
CNC(=O)c1cc(Oc2cc([N+](=O)[O-])c(NC)cc2OC)ccn1.O=Cc1ccc(Br)cc1>O1CCOCC1>CNC(=O)c1cc(Oc2ccc3c(c2)nc(-c2ccc(Br)cc2)n3C)ccn1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-cc10fa94f3074812be93f370e5820499
C1COOOC1.CC(=O)O[BH-](OC(C)=O)OC(C)=O.Nc1ccccc1-c1ccccc1>>C=C(c1ccccc1)C1COC2(CCC(Nc3ccccc3-c3ccccc3)CC2)OO1
O.O1OOCCC1.NC1=C(C=CC=C1)C1=CC=CC=C1.C(C)(=O)O[BH-](OC(C)=O)OC(C)=O.[Na+]>>C1(=C(C=CC=C1)NC1CCC2(OCC(OO2)C(=C)C2=CC=CC=C2)CC1)C1=CC=CC=C1
[CH2:2]1[CH2:9][CH2:10][O:11][O:32][O:31]1.O=[C:1](O[BH-](O[C:8](=O)[CH3:3])O[C:15](=O)[CH3:29])[CH3:13].[NH2:16][c:17]1[cH:18][cH:19][cH:20][cH:21][c:22]1-[c:23]1[cH:24][cH:25][cH:26][cH:27][cH:28]1>>[CH2:1]=[C:2]([c:3]1[cH:4][cH:5][cH:6][cH:7][cH:8]1)[CH:9]1[CH2:10][O:11][C:12]2([CH2:13][CH2:14][CH:15]([NH:16][c:17]3...
C1COOOC1.CC(=O)O[BH-](OC(C)=O)OC(C)=O.Nc1ccccc1-c1ccccc1
C=C(c1ccccc1)C1COC2(CCC(Nc3ccccc3-c3ccccc3)CC2)OO1
null
null
ClCCl
Aromatic Heterocycle Formation
OtherReaction
e1ccf6effe82ed570627042fc7a202dfeff5db514191bfb6c0626713ad8ba185
ab2c134b6353bbc2872cad7da7c653ff912491653702c9701526cbe073308159
C=C(c1ccccc1)C1COC2(CCC(Nc3ccccc3-c3ccccc3)CC2)OO1
O=[C;H0;D3;+0:1](-[CH3;D1;+0:2])-O-[BH-](-O-[C;H0;D3;+0:3](=O)-[CH3;D1;+0:4])-O-[C;H0;D3;+0:5](=O)-[CH3;D1;+0:6].[C:7]1-[CH2;D2;+0:8]-[CH2;D2;+0:9]-[O;H0;D2;+0:10]-[O;H0;D2;+0:11]-[O;H0;D2;+0:12]-1.[NH2;D1;+0:13]-[c:14](:[c:15]):[c:16]>>[CH2;D1;+0:3]=[C;H0;D3;+0:9](-[CH;D3;+0:8]1-[C:7]-[O;H0;D2;+0:12]-[C:17]2(-[C:18]-[...
21.8
[{"value": 21.8, "product": "C1(=C(C=CC=C1)NC1CCC2(OCC(OO2)C(=C)C2=CC=CC=C2)CC1)C1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
To mixture of trioxane 3a (0.50 g, 1.82 mmol) and 2-aminobiphenyl (0.38 g, 2.27 mmol) in dichloromethane (20 ml) acetic acid was added (1 ml) and reaction mixture was stirred at room temp for half an hour. Sodium triacetoxyborohydride (0.58 g, 2.73 mmol) was added slowly and it was stirred for 3 h at room temperature. ...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Peroxide.Peroxide
Ether.Secondary amine.Peroxide.Vinyl
C1COOOC1
c1ccccc1.C1CCC2(CC1)OCCOO2
c1ccccc1.C1CCC2(CC1)OCCOO2.c1ccccc1.c1ccccc1
null
ClCCl
null
null
C1COOOC1.CC(=O)O[BH-](OC(C)=O)OC(C)=O.Nc1ccccc1-c1ccccc1>ClCCl>C=C(c1ccccc1)C1COC2(CCC(Nc3ccccc3-c3ccccc3)CC2)OO1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-8e433fe3a5b94f9cb05d2594a2d623bf
C1COOOC1.CC(=O)O[BH-](OC(C)=O)OC(C)=O.Nc1ccc(-c2ccccc2)cc1>>C=C(c1ccccc1)C1COC2(CCC(Nc3ccc(-c4ccccc4)cc3)CC2)OO1
O.O1OOCCC1.NC1=CC=C(C=C1)C1=CC=CC=C1.C(C)(=O)O[BH-](OC(C)=O)OC(C)=O.[Na+]>>C1(=CC=C(C=C1)NC1CCC2(OCC(OO2)C(=C)C2=CC=CC=C2)CC1)C1=CC=CC=C1
[CH2:2]1[CH2:9][CH2:10][O:11][O:32][O:31]1.O=[C:1](O[BH-](O[C:8](=O)[CH3:3])O[C:15](=O)[CH3:29])[CH3:13].[NH2:16][c:17]1[cH:18][cH:19][c:20](-[c:21]2[cH:22][cH:23][cH:24][cH:25][cH:26]2)[cH:27][cH:28]1>>[CH2:1]=[C:2]([c:3]1[cH:4][cH:5][cH:6][cH:7][cH:8]1)[CH:9]1[CH2:10][O:11][C:12]2([CH2:13][CH2:14][CH:15]([NH:16][c:17...
C1COOOC1.CC(=O)O[BH-](OC(C)=O)OC(C)=O.Nc1ccc(-c2ccccc2)cc1
C=C(c1ccccc1)C1COC2(CCC(Nc3ccc(-c4ccccc4)cc3)CC2)OO1
null
null
ClCCl
Aromatic Heterocycle Formation
OtherReaction
e1ccf6effe82ed570627042fc7a202dfeff5db514191bfb6c0626713ad8ba185
ab2c134b6353bbc2872cad7da7c653ff912491653702c9701526cbe073308159
C=C(c1ccccc1)C1COC2(CCC(Nc3ccc(-c4ccccc4)cc3)CC2)OO1
O=[C;H0;D3;+0:1](-[CH3;D1;+0:2])-O-[BH-](-O-[C;H0;D3;+0:3](=O)-[CH3;D1;+0:4])-O-[C;H0;D3;+0:5](=O)-[CH3;D1;+0:6].[C:7]1-[CH2;D2;+0:8]-[CH2;D2;+0:9]-[O;H0;D2;+0:10]-[O;H0;D2;+0:11]-[O;H0;D2;+0:12]-1.[NH2;D1;+0:13]-[c:14](:[c:15]):[c:16]>>[CH2;D1;+0:3]=[C;H0;D3;+0:9](-[CH;D3;+0:8]1-[C:7]-[O;H0;D2;+0:12]-[C:17]2(-[C:18]-[...
70.5
[{"value": 70.5, "product": "C1(=CC=C(C=C1)NC1CCC2(OCC(OO2)C(=C)C2=CC=CC=C2)CC1)C1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
To a mixture of trioxane 3a (0.40 g, 1.45 mmol) and 4-aminobiphenyl (0.30 g, 1.82 mmol) in dichloromethane (20 ml) acetic acid (1 ml) was added and reaction mixture was stirred at room temp for half an hour. Sodium triacetoxyborohydride (0.46 g, 3.63 mmol) was added slowly and it was stirred for 3 h at room temperature...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Peroxide.Peroxide
Ether.Secondary amine.Peroxide.Vinyl
C1COOOC1
c1ccccc1.C1CCC2(CC1)OCCOO2
c1ccccc1.C1CCC2(CC1)OCCOO2.c1ccccc1.c1ccccc1
null
ClCCl
null
null
C1COOOC1.CC(=O)O[BH-](OC(C)=O)OC(C)=O.Nc1ccc(-c2ccccc2)cc1>ClCCl>C=C(c1ccccc1)C1COC2(CCC(Nc3ccc(-c4ccccc4)cc3)CC2)OO1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-48f2f96693514efc95e18b49d57fb3dd
CCCCO.O=C([O-])[O-].OCCOCCCl.c1ccc2c(c1)N=C(N1CCNCC1)c1ccccc1S2>>O=C(O)/C=C/C(=O)O.OCCOCCN1CCN(C2=Nc3ccccc3Sc3ccccc32)CC1
CCCCO.Cl.N1(CCNCC1)C1=NC2=C(SC3=C1C=CC=C3)C=CC=C2.C(=O)([O-])[O-].[Na+].[Na+].ClCCOCCO.CCCCO>>C=1C=CC2=C(C1)C(=NC=3C=CC=CC3S2)N4CCN(CC4)CCOCCO.C(=C/C(=O)O)\C(=O)O
C[CH2:5][CH2:4][CH2:2][OH:3].[O-:1][C:6](=[O:7])[O-:8].Cl[CH2:14][CH2:13][O:12][CH2:11][CH2:10][OH:9].[NH:15]1[CH2:16][CH2:17][N:18]([C:19]2=[N:20][c:21]3[cH:22][cH:23][cH:24][cH:25][c:26]3[S:27][c:28]3[cH:29][cH:30][cH:31][cH:32][c:33]32)[CH2:34][CH2:35]1>>[O:1]=[C:2]([OH:3])/[CH:4]=[CH:5]/[C:6](=[O:7])[OH:8].[OH:9][C...
CCCCO.O=C([O-])[O-].OCCOCCCl.c1ccc2c(c1)N=C(N1CCNCC1)c1ccccc1S2
O=C(O)/C=C/C(=O)O.OCCOCCN1CCN(C2=Nc3ccccc3Sc3ccccc32)CC1
null
CCCC[N+](CCCC)(CCCC)CCCC.[Br-]
O
C-C Coupling
OtherReaction
966a01ea2948ed1407014be5aefa7081491af4535a35e3de6f886177953b0a8b
fc43d5d9d3dde9473af63a4f418948137903279c5609d3dff4eea459a1927335
c1ccc2c(c1)N=C(N1CCNCC1)c1ccccc1S2
C-[CH2;D2;+0:1]-[CH2;D2;+0:2]-[CH2;D2;+0:3]-[O;D1;H1:4].Cl-[CH2;D2;+0:5]-[C:6]-[#8:7].[#7:8]1-[C:9]-[C:10]-[NH;D2;+0:11]-[C:12]-[C:13]-1.[O-;H0;D1:14]-[C;H0;D3;+0:15](-[O-;H0;D1:16])=[O;D1;H0:17]>>[#8:7]-[C:6]-[CH2;D2;+0:5]-[N;H0;D3;+0:11]1-[C:10]-[C:9]-[#7:8]-[C:13]-[C:12]-1.[O;D1;H0:17]=[C;H0;D3;+0:15](-[OH;D1;+0:16]...
null
[]
25
CELSIUS
null
null
A 100 liter reactor equipped with mechanical stirrer, condenser, and thermometer, was charged with n-BuOH (40.5 L), 11-piperazinyl dibenzo[b,f][1,4]thiazepinehydrochloride (15 kg), Na2CO3 (7.5 kg), TBAB (1.5 kg) and 2-(2-chloroethoxy)ethanol (5.25 L). The mixture was heated to 115° C. during which time a portion of the...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary alcohol.Secondary amine
Carboxylic acid.Carboxylic acid.Tertiary amine
C1CNCC[NH]1
C1C[NH]CC[NH]1
C1C[NH]CC[NH]1.C1=Nc2ccccc2Sc2ccccc21
HCl
CCCC[N+](CCCC)(CCCC)CCCC.[Br-].O
25
null
CCCCO.O=C([O-])[O-].OCCOCCCl.c1ccc2c(c1)N=C(N1CCNCC1)c1ccccc1S2>CCCC[N+](CCCC)(CCCC)CCCC.[Br-].O>O=C(O)/C=C/C(=O)O.OCCOCCN1CCN(C2=Nc3ccccc3Sc3ccccc32)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e3b0a9e08bad46409dd0b43d168b1203
CC1CCN(c2c(-c3c(F)cccc3Cl)c(Cl)nc3ncnn23)CC1.CO>>COc1nc2ncnn2c(NC(C)C)c1-c1c(F)cccc1Cl
CO.ClC1=NC=2N(C(=C1C1=C(C=CC=C1F)Cl)N1CCC(CC1)C)N=CN2.C[O-].[Na+].CO>>COC1=NC=2N(C(=C1C1=C(C=CC=C1F)Cl)NC(C)C)N=CN2
Cl[c:3]1[n:4][c:5]2[n:6][cH:7][n:8][n:9]2[c:10]([N:11]2CC[CH:12]([CH3:13])[CH2:14]C2)[c:15]1-[c:16]1[c:17]([F:18])[cH:19][cH:20][cH:21][c:22]1[Cl:23].[CH3:1][OH:2]>>[CH3:1][O:2][c:3]1[n:4][c:5]2[n:6][cH:7][n:8][n:9]2[c:10]([NH:11][CH:12]([CH3:13])[CH3:14])[c:15]1-[c:16]1[c:17]([F:18])[cH:19][cH:20][cH:21][c:22]1[Cl:23]
CC1CCN(c2c(-c3c(F)cccc3Cl)c(Cl)nc3ncnn23)CC1.CO
COc1nc2ncnn2c(NC(C)C)c1-c1c(F)cccc1Cl
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
ffe2b968e00a78f2945d96650c55db0b64427327a267c0e622b9b7822b8fc548
aa61c717c3decc4b9f621ca66f2e82546c76c601e61592e7a86272dd9f1df4b3
c1ccc(-c2cnc3ncnn3c2)cc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]2:[#7;a:4]:[c:5]:[#7;a:6]:[#7;a:7]:2:[c:8](-[N;H0;D3;+0:9]2-C-C-[CH;D3;+0:10](-[C;D1;H3:11])-[CH2;D2;+0:12]-C-2):[c:13]:1-[c:14].[C;D1;H3:15]-[OH;D1;+0:16]>>[C;D1;H3:11]-[CH;D3;+0:10](-[CH3;D1;+0:12])-[NH;D2;+0:9]-[c:8]1:[#7;a:7]2:[#7;a:6]:[c:5]:[#7;a:4]:[c:3]:2:[#7;a:2]:[c;H0;D3;+0:1](...
null
[]
null
null
null
null
To a solution of 65 mmol 5-chloro-6-(2-chloro-6-fluorophenyl)-7-(4-methylpiperidin-1-yl)-[1,2,4]-triazolo[1,5-α]pyrimidine [cf. EP-A 550 113] in dry methanol 71.5 mmol of a 30% solution of sodium methanolate were added at 20 to 25° C. After having stirred this mixture for about 16 hours at this temperature methanol ws ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Tertiary amine.Methanol
Ether.Secondary amine
c1cnc2ncnn2c1.C1CC[NH]CC1
c1cnc2ncnn2c1
c1cnc2ncnn2c1.c1ccccc1
HCl
null
null
null
CC1CCN(c2c(-c3c(F)cccc3Cl)c(Cl)nc3ncnn23)CC1.CO>>COc1nc2ncnn2c(NC(C)C)c1-c1c(F)cccc1Cl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b2a9f41eff9c4c85a0dfe07c22329aa1
COC1=CC=C2[C@H]3Cc4ccc(OC)c5c4[C@@]2(CCN3C)[C@H]1O5.OO>>COc1ccc2c3c1OC1C(=O)C=C[C@@]4(O)[C@@H](C2)N(C)CC[C@]314
OO.CN1CC[C@]23C4=C5C=CC(=C4O[C@H]2C(=CC=C3[C@H]1C5)OC)OC>>CN1CC[C@]23C4C(=O)C=C[C@]2([C@H]1CC5=C3C(=C(C=C5)OC)O4)O
C[O:12][C:11]1=[CH:13][CH:14]=[C:15]2[C@H:17]3[CH2:18][c:6]4[cH:5][cH:4][c:3]([O:2][CH3:1])[c:8]5[c:7]4[C@:23]2([C@H:10]1[O:9]5)[CH2:22][CH2:21][N:19]3[CH3:20].O[OH:16]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]2[c:7]3[c:8]1[O:9][CH:10]1[C:11](=[O:12])[CH:13]=[CH:14][C@@:15]4([OH:16])[C@@H:17]([CH2:18]2)[N:19]([CH3:20])[CH2:...
COC1=CC=C2[C@H]3Cc4ccc(OC)c5c4[C@@]2(CCN3C)[C@H]1O5.OO
COc1ccc2c3c1OC1C(=O)C=C[C@@]4(O)[C@@H](C2)N(C)CC[C@]314
null
null
null
Acylation
OtherReaction
efa20ff62ebe876e24e2d2de28ad90cbb0a393b571a4ec8e98dc162b5cbea86b
121b0afd551ef6c4ab30f4344a7aba9f94f7d29b2ba3ad55fde8838b38bea58c
O=C1C=CC2[C@H]3Cc4cccc5c4[C@@]2(CCN3)C1O5
C-[O;H0;D2;+0:1]-[C;H0;D3;+0:2]1=[CH;D2;+0:3]-[CH;D2;+0:4]=[C;H0;D3;+0:5]2-[C:6](-[C:7])-[#7:8](-[C;D1;H3:9])-[C:10]-[C:11]-[C:12]-23-[c:13]:[c:14]-[#8:15]-[C@@H;D3;+0:16]-1-3.O-[OH;D1;+0:17]>>[C:7]-[C:6]1-[#7:8](-[C;D1;H3:9])-[C:10]-[C:11]-[C:12]23-[c:13]:[c:14]-[#8:15]-[CH;D3;+0:16]-2-[C;H0;D3;+0:2](=[O;H0;D1;+0:1])-...
null
[]
null
null
3
HOUR
A 0.10 L round bottom flask (RBF) is charged with 18.9 g of formic acid, 9.9 g of water, and 7.8 g of 2-propanol. This mixture is stirred at 20–30° C. for 5 minutes. Into this solution is added 5.0 g of thebaine bitartrate monohydrate. This is stirred magnetically at room temperature for 10 minutes until dissolution is...
10.6084/m9.figshare.5104873.v1
null
Ether.Peroxide.Conjugated diene
Ketone.Tertiary alcohol
C1=C[C@@H]2Oc3cccc4c3[C@@]23CC[NH][C@H](C4)C3=C1
C1=C[C@H]2[C@H]3Cc4cccc5c4[C@@]2(CC[NH]3)C(C1)O5
C1=C[C@H]2[C@H]3Cc4cccc5c4[C@@]2(CC[NH]3)C(C1)O5
HO-
null
null
3
COC1=CC=C2[C@H]3Cc4ccc(OC)c5c4[C@@]2(CCN3C)[C@H]1O5.OO>>COc1ccc2c3c1OC1C(=O)C=C[C@@]4(O)[C@@H](C2)N(C)CC[C@]314
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-1fa2ba475a8c427c8914a6f9aa3a427b
COc1ccc2c3c1OC1C(=O)C=C[C@@]4(O)[C@@H](C2)N(C)CC[C@]314>>COc1ccc2c3c1O[C@H]1C(=O)CC[C@@]4(O)[C@@H](C2)N(C)CC[C@]314
[H][H].[OH-].[Na+].NC(=S)N.[H][H].CN1CC[C@]23C4C(=O)C=C[C@]2([C@H]1CC5=C3C(=C(C=C5)OC)O4)O.P(O)(O)(O)=O.CN1CC[C@]23C4C(=O)C=C[C@]2([C@H]1CC5=C3C(=C(C=C5)OC)O4)O>>CN1CC[C@]23C4=C5C=CC(=C4O[C@H]2C(=O)CC[C@]3([C@H]1C5)O)OC
[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]2[c:7]3[c:8]1[O:9][CH:10]1[C:11](=[O:12])[CH:13]=[CH:14][C@@:15]4([OH:16])[C@@H:17]([CH2:18]2)[N:19]([CH3:20])[CH2:21][CH2:22][C@:23]314>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]2[c:7]3[c:8]1[O:9][C@H:10]1[C:11](=[O:12])[CH2:13][CH2:14][C@@:15]4([OH:16])[C@@H:17]([CH2:18]2)[N:19]([CH3:20])...
COc1ccc2c3c1OC1C(=O)C=C[C@@]4(O)[C@@H](C2)N(C)CC[C@]314
COc1ccc2c3c1O[C@H]1C(=O)CC[C@@]4(O)[C@@H](C2)N(C)CC[C@]314
null
[Pd]
C1CCOC1
Reduction
Hydrogenation (double to single)
752a5e0201ff34934d313f015d6a5a71e40fcc2b623f54907dfade159f526495
0e0db21233797ec1d2a9464a1f32cef94e53e6a41f96d680fa1307067bbf01f2
O=C1CCC2[C@H]3Cc4cccc5c4[C@@]2(CCN3)[C@H]1O5
[#7:1]-[C:2]-[C:3]1(-[O;D1;H1:4])-[C:5]-[C:6](-[#8:7])-[C:8](=[O;D1;H0:9])-[CH;D2;+0:10]=[CH;D2;+0:11]-1>>[#7:1]-[C:2]-[C:3]1(-[O;D1;H1:4])-[C:5]-[C:6](-[#8:7])-[C:8](=[O;D1;H0:9])-[CH2;D2;+0:10]-[CH2;D2;+0:11]-1
91.2
[{"value": 91.0, "product": "CN1CC[C@]23C4=C5C=CC(=C4O[C@H]2C(=O)CC[C@]3([C@H]1C5)O)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 91.2, "product": "CN1CC[C@]23C4=C5C=CC(=C4O[C@H]2C(=O)CC[C@]3([C@H]1C5)O)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A known amount of THF (26.7 g) is charged into a 0.5 L RBF, and 3.05 g of 14-hydroxycodeinone is added into it. With stirring 120 g of aqueous phosphoric acid (1M, 9.8%) is added. The mixture is stirred until the entire solid dissolved. While stirring 40% aqueous sodium hydroxide is added (12.5 g) dropwise over a 30-mi...
10.6084/m9.figshare.5104873.v1
null
Ketone
Ketone
C1=C[C@H]2[C@H]3Cc4cccc5c4[C@@]2(CC[NH]3)C(C1)O5
c1cc2c3c(c1)O[C@H]1CCC[C@H]4[C@@H](C2)[NH]CC[C@]314
c1cc2c3c(c1)O[C@H]1CCC[C@H]4[C@@H](C2)[NH]CC[C@]314
null
[Pd].C1CCOC1
null
null
COc1ccc2c3c1OC1C(=O)C=C[C@@]4(O)[C@@H](C2)N(C)CC[C@]314>[Pd].C1CCOC1>COc1ccc2c3c1O[C@H]1C(=O)CC[C@@]4(O)[C@@H](C2)N(C)CC[C@]314
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4f04d2a2c56b4b278b7210afb01bb875
Cl>>Cl
CN1CC[C@]23C4=C5C=CC(=C4O[C@H]2C(=O)CC[C@]3([C@H]1C5)O)OC.Cl.C(C)O>>CN1CC[C@]23C4=C5C=CC(=C4O[C@H]2C(=O)CC[C@]3([C@H]1C5)O)OC.Cl
[ClH:24]>>[ClH:24]
Cl
Cl
null
null
C(C)O
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
null
[]
null
null
2
HOUR
A known amount of oxycodone (2.80 g) is charged into a 100 mL round-bottom flask equipped with a magnetic stirrer, a reflux condenser, and a thermometer. Into this, 11 g of anhydrous ethanol is added. This is heated to reflux to form a white suspension. Into this hot suspension, 2.75 g of hydrochloride-ethanol solution...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
C(C)O
null
2
Cl>C(C)O>Cl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-190cfc1c9d394de69600f360139a158f
COc1ccc2c3c1OC1C(=O)C=C[C@@]4(O)[C@@H](C2)N(C)CC[C@]314>>COc1ccc2c3c1O[C@H]1C(=O)CC[C@@]4(O)[C@@H](C2)N(C)CC[C@]314
CN1CC[C@]23C4C(=O)C=C[C@]2([C@H]1CC5=C3C(=C(C=C5)OC)O4)O>>CN1CC[C@]23C4=C5C=CC(=C4O[C@H]2C(=O)CC[C@]3([C@H]1C5)O)OC
[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]2[c:7]3[c:8]1[O:9][CH:10]1[C:11](=[O:12])[CH:13]=[CH:14][C@@:15]4([OH:16])[C@@H:17]([CH2:18]2)[N:19]([CH3:20])[CH2:21][CH2:22][C@:23]314>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]2[c:7]3[c:8]1[O:9][C@H:10]1[C:11](=[O:12])[CH2:13][CH2:14][C@@:15]4([OH:16])[C@@H:17]([CH2:18]2)[N:19]([CH3:20])...
COc1ccc2c3c1OC1C(=O)C=C[C@@]4(O)[C@@H](C2)N(C)CC[C@]314
COc1ccc2c3c1O[C@H]1C(=O)CC[C@@]4(O)[C@@H](C2)N(C)CC[C@]314
null
[Pd]
null
Reduction
Hydrogenation (double to single)
752a5e0201ff34934d313f015d6a5a71e40fcc2b623f54907dfade159f526495
0e0db21233797ec1d2a9464a1f32cef94e53e6a41f96d680fa1307067bbf01f2
O=C1CCC2[C@H]3Cc4cccc5c4[C@@]2(CCN3)[C@H]1O5
[#7:1]-[C:2]-[C:3]1(-[O;D1;H1:4])-[C:5]-[C:6](-[#8:7])-[C:8](=[O;D1;H0:9])-[CH;D2;+0:10]=[CH;D2;+0:11]-1>>[#7:1]-[C:2]-[C:3]1(-[O;D1;H1:4])-[C:5]-[C:6](-[#8:7])-[C:8](=[O;D1;H0:9])-[CH2;D2;+0:10]-[CH2;D2;+0:11]-1
85
[{"value": 85.0, "product": "CN1CC[C@]23C4=C5C=CC(=C4O[C@H]2C(=O)CC[C@]3([C@H]1C5)O)OC", "details": "PERCENTYIELD", "is_desired": false}]
null
null
21.5
HOUR
To the solution of 14-hydroxycodeinone produced in Example 14 is added 0.5 g of 5% palladium on carbon, 50% wet. The mixture is hydrogenated at 30 to 40 psi for a period of 18 to 25 hours at ambient temperature. The catalyst is filtered off and is washed with 5 ml of water. The filtrate is cooled to 0–5° C. and with st...
10.6084/m9.figshare.5104873.v1
null
Ketone
Ketone
C1=C[C@H]2[C@H]3Cc4cccc5c4[C@@]2(CC[NH]3)C(C1)O5
c1cc2c3c(c1)O[C@H]1CCC[C@H]4[C@@H](C2)[NH]CC[C@]314
c1cc2c3c(c1)O[C@H]1CCC[C@H]4[C@@H](C2)[NH]CC[C@]314
null
[Pd]
null
21.5
COc1ccc2c3c1OC1C(=O)C=C[C@@]4(O)[C@@H](C2)N(C)CC[C@]314>[Pd]>COc1ccc2c3c1O[C@H]1C(=O)CC[C@@]4(O)[C@@H](C2)N(C)CC[C@]314
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5b665a2b43e14375b34a87ca38617832
Cl>>Cl
Cl.CN1CC[C@]23C4=C5C=CC(=C4O[C@H]2C(=O)CC[C@]3([C@H]1C5)O)OC.C(C)O>>CN1CC[C@]23C4=C5C=CC(=C4O[C@H]2C(=O)CC[C@]3([C@H]1C5)O)OC.Cl
[ClH:24]>>[ClH:24]
Cl
Cl
null
null
C(C)(C)O
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
85
[{"value": 85.0, "product": "CN1CC[C@]23C4=C5C=CC(=C4O[C@H]2C(=O)CC[C@]3([C@H]1C5)O)OC.Cl", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
8.1 g of oxycodone obtained in Example 15 and 80 ml of ethanol are placed in a 250 ml round-bottomed flask. The mixture is heated to reflux. Into the hot mixture is added 10 ml of a concentrated solution of hydrogen chloride in isopropanol. The mixture is cooled and stirred at 0–5° C. for 1–2 hours. The product is filt...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
C(C)(C)O
null
null
Cl>C(C)(C)O>Cl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-23c53c47db3d41769913a28db1a35118
N#Cc1ccc(-c2ccco2)cc1.NC(=NO)c1ccc(Br)cc1>>N#Cc1ccc(-c2ccc(-c3ccc(C#N)cc3)o2)cc1
BrC1=CC=C(C(N)=NO)C=C1.BrC1=CC=C(C(N)=NO)C=C1.C(#N)C1=CC=C(C=C1)C=1OC=CC1>>C(#N)C1=CC=C(C=C1)C=1OC(=CC1)C1=CC=C(C=C1)C#N
[N:1]#[C:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][o:19]2)[cH:20][cH:21]1.ON=[C:15]([c:14]1[cH:13][cH:12][c:11](Br)[cH:18][cH:17]1)[NH2:16]>>[N:1]#[C:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10](-[c:11]3[cH:12][cH:13][c:14]([C:15]#[N:16])[cH:17][cH:18]3)[o:19]2)[cH:20][cH:21]1
N#Cc1ccc(-c2ccco2)cc1.NC(=NO)c1ccc(Br)cc1
N#Cc1ccc(-c2ccc(-c3ccc(C#N)cc3)o2)cc1
null
null
C(C1=CC=CC=C1)#N
C-C Coupling
OtherReaction
1fa403af87c74b70ddf126f5f3d1d35552536a371b7dca5b886385e7398fd93e
5a322521d2e37b68d2c1cdb2695844665e84a24d702c9cebff9cc44ba3f0b615
c1ccc(-c2ccc(-c3ccccc3)o2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](-[C;H0;D3;+0:5](-[NH2;D1;+0:6])=N-O):[c:7]:[c:8]:1.[#8;a:9]1:[c:10]:[c:11]:[c:12]:[cH;D2;+0:13]:1>>[N;H0;D1;+0:6]#[C;H0;D2;+0:5]-[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:13]2:[#8;a:9]:[c:10]:[c:11]:[c:12]:2):[c:8]:[c:7]:1
null
[]
null
null
null
null
in good yield. In contrast, under N-coupling conditions the benzamidoxime was converted to benzonitrile (Anbazhagan et al., (2002) Tetrahedron Lett. 43: 4221) and attempted Heck coupling of 4-bromobenzamidoxime with 2(4-cyanophenyl)furan yielded 2,5-bis(4-cyanophenyl)furan. Conditions: See reaction.notes.procedure_deta...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine.Oxime
Nitrile
c1ccoc1.c1ccccc1
c1ccoc1.c1ccccc1
c1ccccc1.c1ccoc1.c1ccccc1
HBr
C(C1=CC=CC=C1)#N
null
null
N#Cc1ccc(-c2ccco2)cc1.NC(=NO)c1ccc(Br)cc1>C(C1=CC=CC=C1)#N>N#Cc1ccc(-c2ccc(-c3ccc(C#N)cc3)o2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-74abcbab50d444e0b4279f6817692f42
CC[C@H](C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCCl.[I-]>>CC[C@H](C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCI
ClCOC([C@@H](NC(=O)OC(C)(C)C)[C@@H](C)CC)=O.[I-].[Na+]>>ICOC([C@@H](NC(=O)OC(C)(C)C)[C@@H](C)CC)=O
Cl[CH2:17][O:16][C:14]([C@H:5]([C@H:3]([CH2:2][CH3:1])[CH3:4])[NH:6][C:7](=[O:8])[O:9][C:10]([CH3:11])([CH3:12])[CH3:13])=[O:15].[I-:18]>>[CH3:1][CH2:2][C@H:3]([CH3:4])[C@H:5]([NH:6][C:7](=[O:8])[O:9][C:10]([CH3:11])([CH3:12])[CH3:13])[C:14](=[O:15])[O:16][CH2:17][I:18]
CC[C@H](C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCCl.[I-]
CC[C@H](C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCI
null
null
C(C)#N
Functional Group Interconversion
OtherReaction
10bee13c50a4ba107934328c21250869f883899fc8944cf8a0ebee609aa1691d
fe69d77c5ffecf9aa0236c58528d10fdb0294a434868899e60e585d0629b72f9
null
Cl-[CH2;D2;+0:1]-[#8:2]-[C:3](-[C:4])=[O;D1;H0:5].[I-;H0;D0:6]>>[C:4]-[C:3](=[O;D1;H0:5])-[#8:2]-[CH2;D2;+0:1]-[I;H0;D1;+0:6]
87
[{"value": 87.0, "product": "ICOC([C@@H](NC(=O)OC(C)(C)C)[C@@H](C)CC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
4
HOUR
To a solution of N-BOC-L-isoleucine chloromethyl ester (19.6 g, 70 mmol) in acetonitrile (300 mL), was added sodium iodide (31.5 g, 210 mmol). The solution was stirred for 4 h at 60° C. The resulting suspension was filtered and the filtrate was evaporated. The residue was dissolved in CH2Cl2 and washed with aqueous sod...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester
Primary halide
null
null
null
Other
C(C)#N
60
4
CC[C@H](C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCCl.[I-]>C(C)#N>CC[C@H](C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCI
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-7438d544248847338e40decfde61667a
CC(C)(CO)C(=O)O.CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)O>>CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(C)(C)C(=O)O
C(=O)(OC(C)(C)C)N[C@@H](C(C)C)C(=O)O.C1CCC(CC1)N=C=NC2CCCCC2.CC(C(=O)O)(CO)C.N1=CC=CC=C1>>CC(C(=O)O)(COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O)C
[OH:15][CH2:16][C:17]([CH3:18])([CH3:19])[C:20](=[O:21])[OH:22].O[C:13]([C@H:4]([CH:2]([CH3:1])[CH3:3])[NH:5][C:6](=[O:7])[O:8][C:9]([CH3:10])([CH3:11])[CH3:12])=[O:14]>>[CH3:1][CH:2]([CH3:3])[C@H:4]([NH:5][C:6](=[O:7])[O:8][C:9]([CH3:10])([CH3:11])[CH3:12])[C:13](=[O:14])[O:15][CH2:16][C:17]([CH3:18])([CH3:19])[C:20](...
CC(C)(CO)C(=O)O.CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)O
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(C)(C)C(=O)O
null
CN(C1=CC=NC=C1)C
C(Cl)Cl
Acylation
Esterification of Carboxylic Acids
d9bd78214ee7dbc907e499722ae01849a72d188753963443e5df9fe42c31c43b
3652e761944e8ef7ee40675a156c8ae39909c72166786934d88652debf2ec1ac
null
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[#7:5]-[C:6](=[O;D1;H0:7])-[#8:8]-[C:9](-[C;D1;H3:10])(-[C;D1;H3:11])-[C;D1;H3:12].[O;D1;H0:13]=[C:14](-[O;D1;H1:15])-[C:16]-[C:17]-[OH;D1;+0:18]>>[C:4]-[C:3](-[#7:5]-[C:6](=[O;D1;H0:7])-[#8:8]-[C:9](-[C;D1;H3:10])(-[C;D1;H3:11])-[C;D1;H3:12])-[C;H0;D3;+0:1](=[O;D1;H0:2])-[O...
null
[]
null
null
2
HOUR
N-Boc-L-valine (10.8 g, 50 mmole), 4-dimethylaminopyridine (610 mg, 5 mmole) and DCC (6.18 g, 30 mmole) were dissolved in methylene chloride (100 ml). After stirring for 2 hour the mixture was filtered. To the filtrate were added 2,2-dimethyl-3-hydroxy-propionic acid (3.54 g, 30 mmole) and pyridine (10 ml). After 18 hr...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary alcohol
Ester
null
null
null
HO-
CN(C1=CC=NC=C1)C.C(Cl)Cl
null
2
CC(C)(CO)C(=O)O.CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)O>CN(C1=CC=NC=C1)C.C(Cl)Cl>CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(C)(C)C(=O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ed0635e891984285a69798f36ec59943
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(C)(C)C(=O)O.ClCI>>CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(C)(C)C(=O)OCCl
CC(C(=O)O)(COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O)C.[OH-].C(CCC)[N+](CCCC)(CCCC)CCCC.ClCI>>ClCOC(C(COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O)(C)C)=O
[CH3:1][CH:2]([CH3:3])[C@H:4]([NH:5][C:6](=[O:7])[O:8][C:9]([CH3:10])([CH3:11])[CH3:12])[C:13](=[O:14])[O:15][CH2:16][C:17]([CH3:18])([CH3:19])[C:20](=[O:21])[OH:22].I[CH2:23][Cl:24]>>[CH3:1][CH:2]([CH3:3])[C@H:4]([NH:5][C:6](=[O:7])[O:8][C:9]([CH3:10])([CH3:11])[CH3:12])[C:13](=[O:14])[O:15][CH2:16][C:17]([CH3:18])([C...
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(C)(C)C(=O)O.ClCI
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(C)(C)C(=O)OCCl
null
null
O1CCOCC1
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
2f16a3cac6d3c4085515a42267501b7a0eef68b042dbe72a334a9b3dd1458b44
20b23d23df2ca888376bbfdf646588e67491b315935b071cb9ba310488e4ee8f
null
I-[CH2;D2;+0:1]-[Cl;D1;H0:2].[C:3]-[C:4](=[O;D1;H0:5])-[OH;D1;+0:6]>>[C:3]-[C:4](=[O;D1;H0:5])-[O;H0;D2;+0:6]-[CH2;D2;+0:1]-[Cl;D1;H0:2]
null
[]
null
null
18
HOUR
2,2-dimethyl-3-(N-Boc-L-valyloxy)propionic acid (3.9 g, 12.3 mmole) was dissolved in dioxane (60 ml). To the solution was added tetrabutylammonium hydroxide aqueous solution (40%, 7.78 ml, 12 mmole). The solution was dried in vacuo, and it was coevaporated with toluene for several times. The residue was dissolved in me...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary halide.Carboxylic acid
Primary halide.Ester
null
null
null
HI
O1CCOCC1
null
18
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(C)(C)C(=O)O.ClCI>O1CCOCC1>CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(C)(C)C(=O)OCCl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-097a601cbd594cd3941a4a68eb987caa
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(C)(C)C(=O)OCCl.[I-]>>CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(C)(C)C(=O)OCI
ClCOC(C(COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O)(C)C)=O.[I-].[Na+]>>ICOC(C(COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O)(C)C)=O
Cl[CH2:23][O:22][C:20]([C:17]([CH2:16][O:15][C:13]([C@H:4]([CH:2]([CH3:1])[CH3:3])[NH:5][C:6](=[O:7])[O:8][C:9]([CH3:10])([CH3:11])[CH3:12])=[O:14])([CH3:18])[CH3:19])=[O:21].[I-:24]>>[CH3:1][CH:2]([CH3:3])[C@H:4]([NH:5][C:6](=[O:7])[O:8][C:9]([CH3:10])([CH3:11])[CH3:12])[C:13](=[O:14])[O:15][CH2:16][C:17]([CH3:18])([C...
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(C)(C)C(=O)OCCl.[I-]
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(C)(C)C(=O)OCI
null
null
C(C)#N
Functional Group Interconversion
OtherReaction
10bee13c50a4ba107934328c21250869f883899fc8944cf8a0ebee609aa1691d
fe69d77c5ffecf9aa0236c58528d10fdb0294a434868899e60e585d0629b72f9
null
Cl-[CH2;D2;+0:1]-[#8:2]-[C:3](-[C:4])=[O;D1;H0:5].[I-;H0;D0:6]>>[C:4]-[C:3](=[O;D1;H0:5])-[#8:2]-[CH2;D2;+0:1]-[I;H0;D1;+0:6]
94.9
[{"value": 94.9, "product": "ICOC(C(COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O)(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
2,2-Dimethyl-3-(N-Boc-L-valyloxy)propionic acid chloromethyl ester (3.6 g, 10 mmole) was dissolved in acetonitrile (50 ml). Sodium iodide (2.1 g, 14 mmole) was added to the solution. After reaction at 70° C. for 2 hr, the reaction mixture was filtered and the residue was dissolved in methylene chloride (20 ml) and refi...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester
Primary halide
null
null
null
Other
C(C)#N
null
null
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(C)(C)C(=O)OCCl.[I-]>C(C)#N>CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(C)(C)C(=O)OCI
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-73befd23f9934808883731425e70cde4
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCC(COC(=O)[C@@H](NC(=O)OCc1ccccc1)C(C)C)CC(=O)O.ClCI>>CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCC(COC(=O)[C@@H](NC(=O)OCc1ccccc1)C(C)C)CC(=O)OCCl
C(=O)(OCC1=CC=CC=C1)N[C@@H](C(C)C)C(=O)OCC(CC(=O)O)COC([C@@H](NC(=O)OCC1=CC=CC=C1)C(C)C)=O.[OH-].C(CCC)[N+](CCCC)(CCCC)CCCC.ClCI>>ClCOC(CC(COC([C@@H](NC(=O)OCC1=CC=CC=C1)C(C)C)=O)COC([C@@H](NC(=O)OCC1=CC=CC=C1)C(C)C)=O)=O
[CH3:1][CH:2]([CH3:3])[C@H:4]([NH:5][C:6](=[O:7])[O:8][CH2:9][c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1)[C:16](=[O:17])[O:18][CH2:19][CH:20]([CH2:21][O:22][C:23](=[O:24])[C@@H:25]([NH:26][C:27](=[O:28])[O:29][CH2:30][c:31]1[cH:32][cH:33][cH:34][cH:35][cH:36]1)[CH:37]([CH3:38])[CH3:39])[CH2:40][C:41](=[O:42])[OH:43].I[...
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCC(COC(=O)[C@@H](NC(=O)OCc1ccccc1)C(C)C)CC(=O)O.ClCI
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCC(COC(=O)[C@@H](NC(=O)OCc1ccccc1)C(C)C)CC(=O)OCCl
null
null
O1CCOCC1
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
2f16a3cac6d3c4085515a42267501b7a0eef68b042dbe72a334a9b3dd1458b44
20b23d23df2ca888376bbfdf646588e67491b315935b071cb9ba310488e4ee8f
O=C(CNC(=O)OCc1ccccc1)OCCCOC(=O)CNC(=O)OCc1ccccc1
I-[CH2;D2;+0:1]-[Cl;D1;H0:2].[C:3]-[C:4](=[O;D1;H0:5])-[OH;D1;+0:6]>>[C:3]-[C:4](=[O;D1;H0:5])-[O;H0;D2;+0:6]-[CH2;D2;+0:1]-[Cl;D1;H0:2]
null
[]
null
null
null
null
3,3-bis (N-CBz-L-valyloxymethyl)-propionic acid (3 g, 5 mmole) was dissolved in dioxane (20 ml). To the solution was added tetrabutylammonium hydroxide aqueous solution (40%, 3.11 ml, 4.8 mmole). The solution was dried in vacuo, and it was coevaporated with toluene several times. The residue was dissolved in methylene ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary halide.Carboxylic acid
Primary halide.Ester
null
null
c1ccccc1.c1ccccc1
HI
O1CCOCC1
null
null
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCC(COC(=O)[C@@H](NC(=O)OCc1ccccc1)C(C)C)CC(=O)O.ClCI>O1CCOCC1>CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCC(COC(=O)[C@@H](NC(=O)OCc1ccccc1)C(C)C)CC(=O)OCCl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-40bb33a7a90c41e19c53a6da20d2af1b
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCC(COC(=O)[C@@H](NC(=O)OCc1ccccc1)C(C)C)CC(=O)OCCl.[I-]>>CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCC(COC(=O)[C@@H](NC(=O)OCc1ccccc1)C(C)C)CC(=O)OCI
ClCOC(CC(COC([C@@H](NC(=O)OCC1=CC=CC=C1)C(C)C)=O)COC([C@@H](NC(=O)OCC1=CC=CC=C1)C(C)C)=O)=O.[I-].[Na+]>>ICOC(CC(COC([C@@H](NC(=O)OCC1=CC=CC=C1)C(C)C)=O)COC([C@@H](NC(=O)OCC1=CC=CC=C1)C(C)C)=O)=O
Cl[CH2:44][O:43][C:41]([CH2:40][CH:20]([CH2:19][O:18][C:16]([C@H:4]([CH:2]([CH3:1])[CH3:3])[NH:5][C:6](=[O:7])[O:8][CH2:9][c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1)=[O:17])[CH2:21][O:22][C:23](=[O:24])[C@@H:25]([NH:26][C:27](=[O:28])[O:29][CH2:30][c:31]1[cH:32][cH:33][cH:34][cH:35][cH:36]1)[CH:37]([CH3:38])[CH3:39])=...
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCC(COC(=O)[C@@H](NC(=O)OCc1ccccc1)C(C)C)CC(=O)OCCl.[I-]
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCC(COC(=O)[C@@H](NC(=O)OCc1ccccc1)C(C)C)CC(=O)OCI
null
null
C(C)#N
Functional Group Interconversion
OtherReaction
10bee13c50a4ba107934328c21250869f883899fc8944cf8a0ebee609aa1691d
fe69d77c5ffecf9aa0236c58528d10fdb0294a434868899e60e585d0629b72f9
O=C(CNC(=O)OCc1ccccc1)OCCCOC(=O)CNC(=O)OCc1ccccc1
Cl-[CH2;D2;+0:1]-[#8:2]-[C:3](-[C:4])=[O;D1;H0:5].[I-;H0;D0:6]>>[C:4]-[C:3](=[O;D1;H0:5])-[#8:2]-[CH2;D2;+0:1]-[I;H0;D1;+0:6]
null
[]
null
null
null
null
3,3-bis (N-CBz-L-valyloxymethyl)-propionic acid chloromethyl ester (900 mg, 1.38 mmole) was dissolved in acetonitrile (5 ml). Sodium iodide (289 mg, 1.93 mmole) was added to the solution. After reaction at 70° C. for 3 hr, the reaction mixture was filtered and the residue was dissolved in methylene chloride (5 ml) and ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester
Primary halide
null
null
c1ccccc1.c1ccccc1
Other
C(C)#N
null
null
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCC(COC(=O)[C@@H](NC(=O)OCc1ccccc1)C(C)C)CC(=O)OCCl.[I-]>C(C)#N>CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCC(COC(=O)[C@@H](NC(=O)OCc1ccccc1)C(C)C)CC(=O)OCI
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-00c0d255c13b4f788d44e347479860d8
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCCOC(=O)OCCl.[I-]>>CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCCOC(=O)OCI
C(=O)(OCC1=CC=CC=C1)N[C@@H](C(C)C)C(=O)OCCOC(=O)OCCl.[I-].[Na+]>>C(=O)(OCC1=CC=CC=C1)N[C@@H](C(C)C)C(=O)OCCOC(=O)OCI
Cl[CH2:25][O:24][C:22]([O:21][CH2:20][CH2:19][O:18][C:16]([C@H:4]([CH:2]([CH3:1])[CH3:3])[NH:5][C:6](=[O:7])[O:8][CH2:9][c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1)=[O:17])=[O:23].[I-:26]>>[CH3:1][CH:2]([CH3:3])[C@H:4]([NH:5][C:6](=[O:7])[O:8][CH2:9][c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1)[C:16](=[O:17])[O:18][CH2:...
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCCOC(=O)OCCl.[I-]
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCCOC(=O)OCI
null
null
C(C)#N
Functional Group Interconversion
OtherReaction
22e4ae0c85daffd0078fd40b928ca1a4ed497239b66c1b767f5c2602965f1e0a
e5953f4c2f3e929ebd5c80667db5cd8a1df5fb6bd8f8f4de947f99af74ff7227
c1ccccc1
Cl-[CH2;D2;+0:1]-[#8:2]-[C:3](-[#8:4])=[O;D1;H0:5].[I-;H0;D0:6]>>[#8:4]-[C:3](=[O;D1;H0:5])-[#8:2]-[CH2;D2;+0:1]-[I;H0;D1;+0:6]
null
[]
null
null
null
null
2-(N-CBz-L-valyloxy)ethoxycarbonyloxymethyl chloride (1.16 g, 3 mmole) was dissolved in acetonitrile (10 ml). Sodium iodide (630 g, 4.2 mmole) was added to the solution. After reaction at 65° C. for 2.5 hr, the reaction mixture was cooled down to room temperature and filtered and the residue was dissolved in methylene ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Carbonic Ester
Primary halide
null
null
c1ccccc1
Other
C(C)#N
null
null
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCCOC(=O)OCCl.[I-]>C(C)#N>CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCCOC(=O)OCI
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5055b63534954acc80348260aa3b9b65
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)O.CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(O)CO>>CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(O)COC(=O)[C@@H](NC(=O)OC(C)(C)C)C(C)C
C(C)(C)(C)OC(=O)N[C@@H](C(C)C)C(=O)OCC(O)CO.C(=O)(OC(C)(C)C)N[C@@H](C(C)C)C(=O)O.C1CCC(CC1)N=C=NC2CCCCC2>>C(C)(C)(C)OC(=O)N[C@@H](C(C)C)C(=O)OCC(O)COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O
O[C:21](=[O:22])[C@@H:23]([NH:24][C:25](=[O:26])[O:27][C:28]([CH3:29])([CH3:30])[CH3:31])[CH:32]([CH3:33])[CH3:34].[CH3:1][CH:2]([CH3:3])[C@H:4]([NH:5][C:6](=[O:7])[O:8][C:9]([CH3:10])([CH3:11])[CH3:12])[C:13](=[O:14])[O:15][CH2:16][CH:17]([OH:18])[CH2:19][OH:20]>>[CH3:1][CH:2]([CH3:3])[C@H:4]([NH:5][C:6](=[O:7])[O:8][...
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)O.CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(O)CO
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(O)COC(=O)[C@@H](NC(=O)OC(C)(C)C)C(C)C
null
CN(C)C=1C=CN=CC1
CN(C)C=O.C(Cl)Cl
Acylation
Esterification of Carboxylic Acids
d9bd78214ee7dbc907e499722ae01849a72d188753963443e5df9fe42c31c43b
3652e761944e8ef7ee40675a156c8ae39909c72166786934d88652debf2ec1ac
null
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[#7:5]-[C:6](=[O;D1;H0:7])-[#8:8]-[C:9](-[C;D1;H3:10])(-[C;D1;H3:11])-[C;D1;H3:12].[C:13]-[C:14]-[OH;D1;+0:15]>>[C:13]-[C:14]-[O;H0;D2;+0:15]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[#7:5]-[C:6](=[O;D1;H0:7])-[#8:8]-[C:9](-[C;D1;H3:10])(-[C;D1;H3:11])-[C;D1;H3:12]
49
[{"value": 49.0, "product": "C(C)(C)(C)OC(=O)N[C@@H](C(C)C)C(=O)OCC(O)COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 49.0, "product": "C(C)(C)(C)OC(=O)N[C@@H](C(C)C)C(=O)OCC(O)COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false...
null
null
null
null
1-O-(N-tert-butoxycarbonyl-L-valyl)glycerol (17.95 g. 61.6 mmol), Boc-L-valine (6.69 g, 30.8 mmol), DMAP (0.38 g, 3.1 mmol), and DCC (7.10 g, 34.4 mmol) in 240 mL CH2Cl2 and 60 mL DMF were stirred at rt under N2 for 18 h. The reaction mixture was filtered, concentrated under vacuum, and redissolved in 200 mL EtOAc. The...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary alcohol
Ester
null
null
null
HO-
CN(C)C=1C=CN=CC1.CN(C)C=O.C(Cl)Cl
null
null
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)O.CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(O)CO>CN(C)C=1C=CN=CC1.CN(C)C=O.C(Cl)Cl>CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(O)COC(=O)[C@@H](NC(=O)OC(C)(C)C)C(C)C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d739aa045e2e4984bbcf85756bd2cf59
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(O)COC(=O)[C@@H](NC(=O)OC(C)(C)C)C(C)C.O=C(Cl)OCCl>>CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(COC(=O)[C@@H](NC(=O)OC(C)(C)C)C(C)C)OC(=O)OCCl
ClC(=O)OCCl.C(C)(C)(C)OC(=O)N[C@@H](C(C)C)C(=O)OCC(O)COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O.N1=CC=CC=C1>>ClCOC(=O)OC(COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O)COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O
[CH3:1][CH:2]([CH3:3])[C@H:4]([NH:5][C:6](=[O:7])[O:8][C:9]([CH3:10])([CH3:11])[CH3:12])[C:13](=[O:14])[O:15][CH2:16][CH:17]([CH2:18][O:19][C:20](=[O:21])[C@@H:22]([NH:23][C:24](=[O:25])[O:26][C:27]([CH3:28])([CH3:29])[CH3:30])[CH:31]([CH3:32])[CH3:33])[OH:34].Cl[C:35](=[O:36])[O:37][CH2:38][Cl:39]>>[CH3:1][CH:2]([CH3:...
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(O)COC(=O)[C@@H](NC(=O)OC(C)(C)C)C(C)C.O=C(Cl)OCCl
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(COC(=O)[C@@H](NC(=O)OC(C)(C)C)C(C)C)OC(=O)OCCl
null
null
C(Cl)Cl
Acylation
Schotten-Baumann to ester
16a18aa130cea39a3a662ee8b6057b54f71a5546be78b0c40ff9ad2c1213d664
75f277925c316017cfa5d00758bde92cc568ffecb2651aae6fab24b6daa74c11
null
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C:4].[C:5]-[C:6](-[C:7])-[OH;D1;+0:8]>>[C:5]-[C:6](-[C:7])-[O;H0;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C:4]
93.1
[{"value": 93.0, "product": "ClCOC(=O)OC(COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O)COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 93.1, "product": "ClCOC(=O)OC(COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O)COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_d...
null
null
45
MINUTE
Chloromethyl chloroformate (2.70 mL, 30 mmol) was added to a solution of 1,3-di-O-(N-tert-butoxycarbonyl-L-valyl)glycerol (7.27 g, 14.8 mmol) and pyridine (7.2 mL, 89 mmol) in 60 mL dry CH2Cl2, in an ice bath, under N2. After stirring for 1 h 45 min, the reaction mixture was diluted with 100 mL CH2Cl2 and washed with 4...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Ether.Secondary alcohol
Carbonic Ester
null
null
null
HCl
C(Cl)Cl
null
0.75
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(O)COC(=O)[C@@H](NC(=O)OC(C)(C)C)C(C)C.O=C(Cl)OCCl>C(Cl)Cl>CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(COC(=O)[C@@H](NC(=O)OC(C)(C)C)C(C)C)OC(=O)OCCl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-1b60864acca840c38135439a12de4209
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(COC(=O)[C@@H](NC(=O)OC(C)(C)C)C(C)C)OC(=O)OCCl.[I-]>>CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(COC(=O)[C@@H](NC(=O)OC(C)(C)C)C(C)C)OC(=O)OCI
ClCOC(=O)OC(COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O)COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O.[Na+].[I-]>>ICOC(=O)OC(COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O)COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O
Cl[CH2:38][O:37][C:35]([O:34][CH:17]([CH2:16][O:15][C:13]([C@H:4]([CH:2]([CH3:1])[CH3:3])[NH:5][C:6](=[O:7])[O:8][C:9]([CH3:10])([CH3:11])[CH3:12])=[O:14])[CH2:18][O:19][C:20](=[O:21])[C@@H:22]([NH:23][C:24](=[O:25])[O:26][C:27]([CH3:28])([CH3:29])[CH3:30])[CH:31]([CH3:32])[CH3:33])=[O:36].[I-:39]>>[CH3:1][CH:2]([CH3:3...
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(COC(=O)[C@@H](NC(=O)OC(C)(C)C)C(C)C)OC(=O)OCCl.[I-]
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(COC(=O)[C@@H](NC(=O)OC(C)(C)C)C(C)C)OC(=O)OCI
null
null
null
Functional Group Interconversion
OtherReaction
22e4ae0c85daffd0078fd40b928ca1a4ed497239b66c1b767f5c2602965f1e0a
e5953f4c2f3e929ebd5c80667db5cd8a1df5fb6bd8f8f4de947f99af74ff7227
null
Cl-[CH2;D2;+0:1]-[#8:2]-[C:3](-[#8:4])=[O;D1;H0:5].[I-;H0;D0:6]>>[#8:4]-[C:3](=[O;D1;H0:5])-[#8:2]-[CH2;D2;+0:1]-[I;H0;D1;+0:6]
92
[{"value": 92.0, "product": "ICOC(=O)OC(COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O)COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 92.0, "product": "ICOC(=O)OC(COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O)COC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_des...
80
CELSIUS
null
null
A solution of 2-O-chloromethoxycarbonyl-1,3-di-O-(N-tert-butoxycarbonyl-L-valyl)propane-1,2,3-triol (7.86 g, 13.5 mmol) and NaI (8.09 g, 54.0 mmol) in 135 mL dry acetonitirile was refluxed at 80° C. for 4 h under N2. The reaction mixture was concentrated under vacuum, and then partitioned between 150 mL diethyl ether a...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Carbonic Ester
Primary halide
null
null
null
Other
null
80
null
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(COC(=O)[C@@H](NC(=O)OC(C)(C)C)C(C)C)OC(=O)OCCl.[I-]>>CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCC(COC(=O)[C@@H](NC(=O)OC(C)(C)C)C(C)C)OC(=O)OCI
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0560d91a7a5847519b31a7e0a7966b24
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCC(OC(=O)[C@@H](NC(=O)OCc1ccccc1)C(C)C)C(=O)OC(C)(C)C>>CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCC(OC(=O)[C@@H](NC(=O)OCc1ccccc1)C(C)C)C(=O)O
C(C)(C)(C)OC(C(COC([C@@H](NC(=O)OCC1=CC=CC=C1)C(C)C)=O)OC([C@@H](NC(=O)OCC1=CC=CC=C1)C(C)C)=O)=O.FC(C(=O)O)(F)F>>C(=O)(OCC1=CC=CC=C1)N[C@@H](C(C)C)C(=O)OC(C(=O)O)COC([C@@H](NC(=O)OCC1=CC=CC=C1)C(C)C)=O
CC(C)(C)[O:41][C:39]([CH:20]([CH2:19][O:18][C:16]([C@H:4]([CH:2]([CH3:1])[CH3:3])[NH:5][C:6](=[O:7])[O:8][CH2:9][c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1)=[O:17])[O:21][C:22](=[O:23])[C@@H:24]([NH:25][C:26](=[O:27])[O:28][CH2:29][c:30]1[cH:31][cH:32][cH:33][cH:34][cH:35]1)[CH:36]([CH3:37])[CH3:38])=[O:40]>>[CH3:1][CH...
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCC(OC(=O)[C@@H](NC(=O)OCc1ccccc1)C(C)C)C(=O)OC(C)(C)C
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCC(OC(=O)[C@@H](NC(=O)OCc1ccccc1)C(C)C)C(=O)O
null
null
ClCCl
Deprotection
Deprotection of carboxylic acid
152e5537e48c95b4a3e767536b0f9f68d1308e5f484070828ab5ed951805157a
7f019d4cfe9b3036d0a2d3a3209aa0e1fcb05418ebee15a4be5e125d315d5f01
O=C(CNC(=O)OCc1ccccc1)OCCOC(=O)CNC(=O)OCc1ccccc1
C-C(-C)(-C)-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
null
[]
null
null
5
HOUR
To a solution of t-butyl -2,3-bis-(N-CBz-L-valyloxy)-propionate (7.2 g, 11.4 mmole) in dichloromethane (25 ml) was added trifluoroacetic acid (25 ml) and the solution was stirred for five hours at room temperature. The solution was evaporated under reduced pressure and coevaporated two times with toluene. The product w...
10.6084/m9.figshare.5104873.v1
null
Ester.Boc
Carboxylic acid
null
null
c1ccccc1.c1ccccc1
Other
ClCCl
null
5
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCC(OC(=O)[C@@H](NC(=O)OCc1ccccc1)C(C)C)C(=O)OC(C)(C)C>ClCCl>CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)OCC(OC(=O)[C@@H](NC(=O)OCc1ccccc1)C(C)C)C(=O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4078ad561ddb47a59a34b89ace3ee1ca
COc1ccc(CCl)cc1.C[C@H](O)C(=O)O>>COc1ccc(COC(=O)[C@H](C)O)cc1
COC1=CC=C(CCl)C=C1.O[C@H](C(=O)O)C.CC(C)([O-])C.[K+]>>O[C@H](C(=O)OCC1=CC=C(C=C1)OC)C
Cl[CH2:7][c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:15][cH:14]1.[OH:8][C:9](=[O:10])[C@H:11]([CH3:12])[OH:13]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][O:8][C:9](=[O:10])[C@H:11]([CH3:12])[OH:13])[cH:14][cH:15]1
COc1ccc(CCl)cc1.C[C@H](O)C(=O)O
COc1ccc(COC(=O)[C@H](C)O)cc1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
06c4f868ad4646eea8208ecb83f54ca035dd62d04f0d8101641a4f487f2c695c
8446834f0edd1e71a2dcaffc09b80c7367abf3407263a8998354a2d20c1766bb
c1ccccc1
Cl-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[C:5]-[C:6](=[O;D1;H0:7])-[OH;D1;+0:8]>>[C:5]-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
25
CELSIUS
1
HOUR
To a stirred solution of (S)(+)2 hydroxypropionic acid (9.0 g, 100 mmole) in 100 ml dry DMF was added potassium tert-butoxide (12.34 g, 110 mmole) and the mixture was stirred for one hour at 25° C. 4-Methoxybenzyl chloride (18.8 g 120 mmole) was added and the mixture was stirred for six hours at 60° C. The mixture was ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Carboxylic acid
Ester
null
null
c1ccccc1
HCl
CN(C)C=O
25
1
COc1ccc(CCl)cc1.C[C@H](O)C(=O)O>CN(C)C=O>COc1ccc(COC(=O)[C@H](C)O)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-305a509630c049e1b60a23777bf2b192
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)O.COc1ccc(COC(=O)[C@H](C)O)cc1>>COc1ccc(COC(=O)[C@H](C)OC(=O)[C@@H](NC(=O)OCc2ccccc2)C(C)C)cc1
O[C@H](C(=O)OCC1=CC=C(C=C1)OC)C.C(=O)(OCC1=CC=CC=C1)N[C@@H](C(C)C)C(=O)O.C1CCC(CC1)N=C=NC2CCCCC2>>C(=O)(OCC1=CC=CC=C1)N[C@@H](C(C)C)C(=O)O[C@H](C(=O)OCC1=CC=C(C=C1)OC)C
O[C:14](=[O:15])[C@@H:16]([NH:17][C:18](=[O:19])[O:20][CH2:21][c:22]1[cH:23][cH:24][cH:25][cH:26][cH:27]1)[CH:28]([CH3:29])[CH3:30].[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][O:8][C:9](=[O:10])[C@H:11]([CH3:12])[OH:13])[cH:31][cH:32]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][O:8][C:9](=[O:10])[C@H:11]([CH3:12])[O:...
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)O.COc1ccc(COC(=O)[C@H](C)O)cc1
COc1ccc(COC(=O)[C@H](C)OC(=O)[C@@H](NC(=O)OCc2ccccc2)C(C)C)cc1
null
CN(C)C=1C=CN=CC1
ClCCl
Acylation
Esterification of Carboxylic Acids
e916c5b009194e30c618975b40d7a233bfcf81339e65494c4e365f67cc5e011d
12ba7405a548c6b1674f05065819c74f53f1b6165cd54e84e1f2f208042fe660
O=C(CNC(=O)OCc1ccccc1)OCC(=O)OCc1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[#7:5]-[C:6]=[O;D1;H0:7].[C:8]-[#8:9]-[C:10](=[O;D1;H0:11])-[C:12](-[C;D1;H3:13])-[OH;D1;+0:14]>>[C:4]-[C:3](-[#7:5]-[C:6]=[O;D1;H0:7])-[C;H0;D3;+0:1](=[O;D1;H0:2])-[O;H0;D2;+0:14]-[C:12](-[C;D1;H3:13])-[C:10](=[O;D1;H0:11])-[#8:9]-[C:8]
null
[]
null
null
8
HOUR
To a solution of 4-methoxybenzyl (S)-(+)-2-hydroxypropionate (7.6 g, 36 mmole), N-CBZ-L-valine (10.05 g, 40 mmole) and DMAP (0.98 g, 8 mmole) in 150 ml dichloromethane was added a solution of DCC (8.3 g, 40 mmole) and the mixture was stirred overnight at room temperature. The mixture was cooled to about 5° C. and the u...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary alcohol
Ester
null
null
c1ccccc1.c1ccccc1
HO-
CN(C)C=1C=CN=CC1.ClCCl
null
8
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)O.COc1ccc(COC(=O)[C@H](C)O)cc1>CN(C)C=1C=CN=CC1.ClCCl>COc1ccc(COC(=O)[C@H](C)OC(=O)[C@@H](NC(=O)OCc2ccccc2)C(C)C)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-7840512745e0442c8c468c30f3c605b0
COc1ccc(COC(=O)[C@H](C)OC(=O)[C@@H](NC(=O)OCc2ccccc2)C(C)C)cc1>>CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)O[C@@H](C)C(=O)O
C(=O)(OCC1=CC=CC=C1)N[C@@H](C(C)C)C(=O)O[C@H](C(=O)OCC1=CC=C(C=C1)OC)C.FC(C(=O)O)(F)F>>C(=O)(OCC1=CC=CC=C1)N[C@@H](C(C)C)C(=O)O[C@H](C(=O)O)C
COc1ccc(C[O:23][C:21]([C@@H:19]([O:18][C:16]([C@H:4]([CH:2]([CH3:1])[CH3:3])[NH:5][C:6](=[O:7])[O:8][CH2:9][c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)=[O:17])[CH3:20])=[O:22])cc1>>[CH3:1][CH:2]([CH3:3])[C@H:4]([NH:5][C:6](=[O:7])[O:8][CH2:9][c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1)[C:16](=[O:17])[O:18][C@@H:19]([CH...
COc1ccc(COC(=O)[C@H](C)OC(=O)[C@@H](NC(=O)OCc2ccccc2)C(C)C)cc1
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)O[C@@H](C)C(=O)O
null
null
ClCCl
Reduction
Ester saponification (alkyl deprotection)
af4a00273af84ecb3074b1842201a78a3aac9a41d2050132ad8c8c1c9d796dee
8d997f8b7994d8c9cf23425771b3f80d4d4830ac4e3d6552f381db244a5a65c5
c1ccccc1
C-O-c1:c:c:c(-C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]):c:c:1>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
null
[]
null
null
5
HOUR
To a solution of 4-methoxybenzyl (S)-(+)-2-(N-CBz-L-valyloxy)propionate (14.0 g, 31.5 mmole) in dichloromethane (50 ml) was added trifluoroacetic acid (25 ml) and the solution was stirred for five hours at room temperature. The solution was evaporated under reduced pressure and coevaporated two times with toluene. The ...
10.6084/m9.figshare.5104873.v1
null
Ester.Ether
Carboxylic acid
c1ccccc1
null
c1ccccc1
HO-
ClCCl
null
5
COc1ccc(COC(=O)[C@H](C)OC(=O)[C@@H](NC(=O)OCc2ccccc2)C(C)C)cc1>ClCCl>CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)O[C@@H](C)C(=O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-456261c7dad64f4b82b109c7e26a8345
CC(O)C(=O)O.COc1ccc(CCl)cc1>>COc1ccc(COC(=O)C(C)O)cc1
COC1=CC=C(CCl)C=C1.OC(C(=O)O)C.CC(C)([O-])C.[K+]>>OC(C(=O)OCC1=CC=C(C=C1)OC)C
[OH:8][C:9](=[O:10])[CH:11]([CH3:12])[OH:13].Cl[CH2:7][c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:15][cH:14]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][O:8][C:9](=[O:10])[CH:11]([CH3:12])[OH:13])[cH:14][cH:15]1
CC(O)C(=O)O.COc1ccc(CCl)cc1
COc1ccc(COC(=O)C(C)O)cc1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
06c4f868ad4646eea8208ecb83f54ca035dd62d04f0d8101641a4f487f2c695c
8446834f0edd1e71a2dcaffc09b80c7367abf3407263a8998354a2d20c1766bb
c1ccccc1
Cl-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[C:5]-[C:6](=[O;D1;H0:7])-[OH;D1;+0:8]>>[C:5]-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
60
CELSIUS
1
HOUR
To a stirred solution of DL -2 hydroxypropionic acid (9.0 g, 100 mmole) in 100 ml dry DMF was added potassium tert-butoxide (12.34 g, 110 mmole) and the mixture was stirred for one hour at 60° C. 4-methoxybenzyl chloride (18.8 g 120 mmole) was added and the mixture was stirred for eight hours at 60° C. The mixture was ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Carboxylic acid
Ester
null
null
c1ccccc1
HCl
CN(C)C=O
60
1
CC(O)C(=O)O.COc1ccc(CCl)cc1>CN(C)C=O>COc1ccc(COC(=O)C(C)O)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-edeb5c0877c6433683ae07456348746b
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)O.COc1ccc(COC(=O)C(C)O)cc1>>COc1ccc(COC(=O)C(C)OC(=O)[C@@H](NC(=O)OCc2ccccc2)C(C)C)cc1
OC(C(=O)OCC1=CC=C(C=C1)OC)C.C(=O)(OCC1=CC=CC=C1)N[C@@H](C(C)C)C(=O)O.C1CCC(CC1)N=C=NC2CCCCC2>>C(=O)(OCC1=CC=CC=C1)N[C@@H](C(C)C)C(=O)OC(C(=O)OCC1=CC=C(C=C1)OC)C
O[C:14](=[O:15])[C@@H:16]([NH:17][C:18](=[O:19])[O:20][CH2:21][c:22]1[cH:23][cH:24][cH:25][cH:26][cH:27]1)[CH:28]([CH3:29])[CH3:30].[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][O:8][C:9](=[O:10])[CH:11]([CH3:12])[OH:13])[cH:31][cH:32]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][O:8][C:9](=[O:10])[CH:11]([CH3:12])[O:13...
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)O.COc1ccc(COC(=O)C(C)O)cc1
COc1ccc(COC(=O)C(C)OC(=O)[C@@H](NC(=O)OCc2ccccc2)C(C)C)cc1
null
CN(C)C=1C=CN=CC1
ClCCl
Acylation
Esterification of Carboxylic Acids
e916c5b009194e30c618975b40d7a233bfcf81339e65494c4e365f67cc5e011d
12ba7405a548c6b1674f05065819c74f53f1b6165cd54e84e1f2f208042fe660
O=C(CNC(=O)OCc1ccccc1)OCC(=O)OCc1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[#7:5]-[C:6]=[O;D1;H0:7].[C:8]-[#8:9]-[C:10](=[O;D1;H0:11])-[C:12](-[C;D1;H3:13])-[OH;D1;+0:14]>>[C:4]-[C:3](-[#7:5]-[C:6]=[O;D1;H0:7])-[C;H0;D3;+0:1](=[O;D1;H0:2])-[O;H0;D2;+0:14]-[C:12](-[C;D1;H3:13])-[C:10](=[O;D1;H0:11])-[#8:9]-[C:8]
null
[]
null
null
8
HOUR
To a solution of 4-methoxybenzyl 2-hydroxypropionate (4.2 g, 20 mmole), N-CBZ-L-valine (5.02 g, 20 mmole) and DMAP (0.24 g, 2 mmole) in 100 ml dichloromethane was added a solution of DCC (4.54 g, 22 mmole) and the mixture was stirred overnight at room temperature. The mixture was cooled to 5° C. and the urethane was fi...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary alcohol
Ester
null
null
c1ccccc1.c1ccccc1
HO-
CN(C)C=1C=CN=CC1.ClCCl
null
8
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)O.COc1ccc(COC(=O)C(C)O)cc1>CN(C)C=1C=CN=CC1.ClCCl>COc1ccc(COC(=O)C(C)OC(=O)[C@@H](NC(=O)OCc2ccccc2)C(C)C)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e8eadd3b067844bca8812cc13ec1e10c
COc1ccc(COC(=O)C(C)OC(=O)[C@@H](NC(=O)OCc2ccccc2)C(C)C)cc1>>CC(OC(=O)[C@@H](NC(=O)OCc1ccccc1)C(C)C)C(=O)O
C(=O)(OCC1=CC=CC=C1)N[C@@H](C(C)C)C(=O)OC(C(=O)OCC1=CC=C(C=C1)OC)C.FC(C(=O)O)(F)F>>C(=O)(OCC1=CC=CC=C1)N[C@@H](C(C)C)C(=O)OC(C(=O)O)C
COc1ccc(C[O:23][C:21]([CH:2]([CH3:1])[O:3][C:4](=[O:5])[C@@H:6]([NH:7][C:8](=[O:9])[O:10][CH2:11][c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[CH:18]([CH3:19])[CH3:20])=[O:22])cc1>>[CH3:1][CH:2]([O:3][C:4](=[O:5])[C@@H:6]([NH:7][C:8](=[O:9])[O:10][CH2:11][c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1)[CH:18]([CH3:19])[CH3:...
COc1ccc(COC(=O)C(C)OC(=O)[C@@H](NC(=O)OCc2ccccc2)C(C)C)cc1
CC(OC(=O)[C@@H](NC(=O)OCc1ccccc1)C(C)C)C(=O)O
null
null
ClCCl
Reduction
Ester saponification (alkyl deprotection)
af4a00273af84ecb3074b1842201a78a3aac9a41d2050132ad8c8c1c9d796dee
8d997f8b7994d8c9cf23425771b3f80d4d4830ac4e3d6552f381db244a5a65c5
c1ccccc1
C-O-c1:c:c:c(-C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]):c:c:1>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
null
[]
null
null
1
HOUR
To a solution of 4-methoxybenzyl 2-(N-CBZ-L-valyloxy)-propionate (7.8 g, 17.5 mmole) in dichloromethane (100 ml) was added trifluoroacetic acid (10 ml) and the solution was stirred for one hour at room temperature. The solution was evaporated under reduced pressure and the product was isolated by silica gel column chro...
10.6084/m9.figshare.5104873.v1
null
Ester.Ether
Carboxylic acid
c1ccccc1
null
c1ccccc1
HO-
ClCCl
null
1
COc1ccc(COC(=O)C(C)OC(=O)[C@@H](NC(=O)OCc2ccccc2)C(C)C)cc1>ClCCl>CC(OC(=O)[C@@H](NC(=O)OCc1ccccc1)C(C)C)C(=O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5ea8029c5565435aad47984724f08609
O=C1CCC(=O)O1.OCc1ccccc1>>O=C(O)CCC(=O)OCc1ccccc1
C(CC(O)(C(=O)O)CC(=O)O)(=O)O.C(C1=CC=CC=C1)O.N1=CC=CC=C1.C1(CCC(=O)O1)=O>>C(C1=CC=CC=C1)OC(CCC(=O)O)=O
[O:1]=[C:2]1[O:3][C:6](=[O:7])[CH2:5][CH2:4]1.[OH:8][CH2:9][c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1>>[O:1]=[C:2]([OH:3])[CH2:4][CH2:5][C:6](=[O:7])[O:8][CH2:9][c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1
O=C1CCC(=O)O1.OCc1ccccc1
O=C(O)CCC(=O)OCc1ccccc1
null
CN(C1=CC=NC=C1)C
C(Cl)Cl
Protection
OtherReaction
4d42d7d8bd0730c96932c909b16e8978d1df708884f50ef85240f28185bc7156
270493bb1736fbee778267cc9a23b684a84d6981f75eccd61f548310bd2b7198
c1ccccc1
[O;D1;H0:1]=[C:2]1-[C:3]-[C:4]-[C;H0;D3;+0:5](=[O;D1;H0:6])-[O;H0;D2;+0:7]-1.[OH;D1;+0:8]-[C:9]-[c:10]>>[O;D1;H0:1]=[C:2](-[OH;D1;+0:7])-[C:3]-[C:4]-[C;H0;D3;+0:5](=[O;D1;H0:6])-[O;H0;D2;+0:8]-[C:9]-[c:10]
null
[]
null
null
30
MINUTE
Succinic anhydride (30 g, 300 mmole) was dissolved in methylene chloride (300 ml). To the solution were added benzyl alcohol (10.2 ml, 100 mmole), 4-dimethylaminopyridine (1.22 g, 10 mmole) and pyridine (48 ml). After 3 hours the reaction mixture was poured in to citric acid aqueous solution. The organic phase was conc...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Primary alcohol
Carboxylic acid.Ester
C1CCOC1
null
c1ccccc1
null
CN(C1=CC=NC=C1)C.C(Cl)Cl
null
0.5
O=C1CCC(=O)O1.OCc1ccccc1>CN(C1=CC=NC=C1)C.C(Cl)Cl>O=C(O)CCC(=O)OCc1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a7826aa50cc047a29967dc9daa70be1e
ClCI.O=C(O)CCC(=O)OCc1ccccc1>>O=C(CCC(=O)OCc1ccccc1)OCCl
C(C1=CC=CC=C1)OC(CCC(=O)O)=O.[OH-].C(CCC)[N+](CCCC)(CCCC)CCCC.ClCI>>ClCOC(CCC(=O)OCC1=CC=CC=C1)=O
I[CH2:16][Cl:17].[O:1]=[C:2]([CH2:3][CH2:4][C:5](=[O:6])[O:7][CH2:8][c:9]1[cH:10][cH:11][cH:12][cH:13][cH:14]1)[OH:15]>>[O:1]=[C:2]([CH2:3][CH2:4][C:5](=[O:6])[O:7][CH2:8][c:9]1[cH:10][cH:11][cH:12][cH:13][cH:14]1)[O:15][CH2:16][Cl:17]
ClCI.O=C(O)CCC(=O)OCc1ccccc1
O=C(CCC(=O)OCc1ccccc1)OCCl
null
null
O1CCOCC1
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
2f16a3cac6d3c4085515a42267501b7a0eef68b042dbe72a334a9b3dd1458b44
20b23d23df2ca888376bbfdf646588e67491b315935b071cb9ba310488e4ee8f
c1ccccc1
I-[CH2;D2;+0:1]-[Cl;D1;H0:2].[C:3]-[C:4](=[O;D1;H0:5])-[OH;D1;+0:6]>>[C:3]-[C:4](=[O;D1;H0:5])-[O;H0;D2;+0:6]-[CH2;D2;+0:1]-[Cl;D1;H0:2]
null
[]
null
null
18
HOUR
Succinic acid monobenzyl ester (4.16 g, 20 mmole) was dissolved in dioxane (20 ml). To the solution was added tetrabutylammonium hydroxide aqueous solution (40%, 11.6 ml, 18 mmole). The solution was dried in vacuo and coevaporated with toluene several times. The residue was dissolved in methylene chloride (60 ml) and t...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary halide.Carboxylic acid
Primary halide.Ester
null
null
c1ccccc1
HI
O1CCOCC1
null
18
ClCI.O=C(O)CCC(=O)OCc1ccccc1>O1CCOCC1>O=C(CCC(=O)OCc1ccccc1)OCCl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-6670ce32e0b94bc78f210052339ddcd9
O=C(CCC(=O)OCc1ccccc1)OCCl.[I-]>>O=C(CCC(=O)OCc1ccccc1)OCI
ClCOC(CCC(=O)OCC1=CC=CC=C1)=O.[I-].[Na+]>>ICOC(CCC(=O)OCC1=CC=CC=C1)=O
Cl[CH2:16][O:15][C:2](=[O:1])[CH2:3][CH2:4][C:5](=[O:6])[O:7][CH2:8][c:9]1[cH:10][cH:11][cH:12][cH:13][cH:14]1.[I-:17]>>[O:1]=[C:2]([CH2:3][CH2:4][C:5](=[O:6])[O:7][CH2:8][c:9]1[cH:10][cH:11][cH:12][cH:13][cH:14]1)[O:15][CH2:16][I:17]
O=C(CCC(=O)OCc1ccccc1)OCCl.[I-]
O=C(CCC(=O)OCc1ccccc1)OCI
null
null
C(C)#N
Functional Group Interconversion
OtherReaction
10bee13c50a4ba107934328c21250869f883899fc8944cf8a0ebee609aa1691d
fe69d77c5ffecf9aa0236c58528d10fdb0294a434868899e60e585d0629b72f9
c1ccccc1
Cl-[CH2;D2;+0:1]-[#8:2]-[C:3](-[C:4])=[O;D1;H0:5].[I-;H0;D0:6]>>[C:4]-[C:3](=[O;D1;H0:5])-[#8:2]-[CH2;D2;+0:1]-[I;H0;D1;+0:6]
null
[]
null
null
null
null
3-Benzyloxycarbonylpropionic acid chloromethyl ester (2 g, 1.38 mmole) was dissolved in acetonitrile (30 ml). Sodium iodide (1.6 g, 10.9 mmole) was added to the solution. After reaction at 70° C. for 3 hr, the reaction mixture was filtered and the residue was dissolved in methylene chloride (20 ml) and refiltered. The ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester
Primary halide
null
null
c1ccccc1
Other
C(C)#N
null
null
O=C(CCC(=O)OCc1ccccc1)OCCl.[I-]>C(C)#N>O=C(CCC(=O)OCc1ccccc1)OCI
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-3d76282a1f9143b792bd2547fb2fed39
O=C(O)CCCBr.OCc1ccccc1>>O=C(CCCBr)OCc1ccccc1
C([O-])(O)=O.[Na+].C(C1=CC=CC=C1)O.BrCCCC(=O)O.C(C)N(CC)CC>>C(C1=CC=CC=C1)OC(CCCBr)=O
O[C:2](=[O:1])[CH2:3][CH2:4][CH2:5][Br:6].[OH:7][CH2:8][c:9]1[cH:10][cH:11][cH:12][cH:13][cH:14]1>>[O:1]=[C:2]([CH2:3][CH2:4][CH2:5][Br:6])[O:7][CH2:8][c:9]1[cH:10][cH:11][cH:12][cH:13][cH:14]1
O=C(O)CCCBr.OCc1ccccc1
O=C(CCCBr)OCc1ccccc1
null
null
S(=O)(Cl)Cl
Protection
Esterification of Carboxylic Acids
070670f68a20c1021da94fabee54def4688122fb721af5f52cd5a03630845d0e
0d8a72b7375d91aa7263e766e03a3cb7c4fa91e27abcd590409ff03b98eed690
c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4].[OH;D1;+0:5]-[C:6]-[c:7]>>[C:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[O;H0;D2;+0:5]-[C:6]-[c:7]
null
[]
-50
CELSIUS
4
HOUR
4-bromobutyric acid (10.6 g, 60 mmole) was dissolved in thionyl chloride (20 mml), and the reaction was kept for 4 hr. The solution was evaporated and coevaporated with toluene several times. The residue was redissolved in dichloromethane (120 ml), and then benzyl alcohol (4.14 ml, 40 mmole) was added. The solution was...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary alcohol
Ester
null
null
c1ccccc1
HO-
S(=O)(Cl)Cl
-50
4
O=C(O)CCCBr.OCc1ccccc1>S(=O)(Cl)Cl>O=C(CCCBr)OCc1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-22938041f184471290a132a36fbb3439
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)O.O=C(CCCBr)OCc1ccccc1>>CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCCCC(=O)OCc1ccccc1
C([O-])(O)=O.[Na+].[OH-].C(CCC)[N+](CCCC)(CCCC)CCCC.C(=O)(OC(C)(C)C)N[C@@H](C(C)C)C(=O)O.C(C1=CC=CC=C1)OC(CCCBr)=O>>C(C1=CC=CC=C1)OC(CCCOC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O)=O
[CH3:1][CH:2]([CH3:3])[C@H:4]([NH:5][C:6](=[O:7])[O:8][C:9]([CH3:10])([CH3:11])[CH3:12])[C:13](=[O:14])[OH:15].Br[CH2:16][CH2:17][CH2:18][C:19](=[O:20])[O:21][CH2:22][c:23]1[cH:24][cH:25][cH:26][cH:27][cH:28]1>>[CH3:1][CH:2]([CH3:3])[C@H:4]([NH:5][C:6](=[O:7])[O:8][C:9]([CH3:10])([CH3:11])[CH3:12])[C:13](=[O:14])[O:15]...
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)O.O=C(CCCBr)OCc1ccccc1
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCCCC(=O)OCc1ccccc1
null
null
O1CCOCC1
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
06c4f868ad4646eea8208ecb83f54ca035dd62d04f0d8101641a4f487f2c695c
8446834f0edd1e71a2dcaffc09b80c7367abf3407263a8998354a2d20c1766bb
c1ccccc1
Br-[CH2;D2;+0:1]-[C:2]-[C:3]-[C:4](-[#8:5])=[O;D1;H0:6].[C:7]-[C:8](=[O;D1;H0:9])-[OH;D1;+0:10]>>[#8:5]-[C:4](=[O;D1;H0:6])-[C:3]-[C:2]-[CH2;D2;+0:1]-[O;H0;D2;+0:10]-[C:8](-[C:7])=[O;D1;H0:9]
null
[]
null
null
18
HOUR
N-Boc-L-valine (1.3 g, 6 mmole) was dissolved in dioxane (5 ml). To the solution was added tetrabutylammonium hydroxide aqueous solution (40%, 3.8 ml, 6 mmole), and the solution was evaporated and coevaporated with toluene several times. The residue was dissolved in DMF (15 ml) and 4-bromobutyric acid benzyl ester (1.2...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Carboxylic acid
Ester
null
null
c1ccccc1
HBr
O1CCOCC1
null
18
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)O.O=C(CCCBr)OCc1ccccc1>O1CCOCC1>CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCCCC(=O)OCc1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-018eebc2a02e453fa7802c31187ef152
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCCCC(=O)OCc1ccccc1>>CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCCCC(=O)O
C(C1=CC=CC=C1)OC(CCCOC([C@@H](NC(=O)OC(C)(C)C)C(C)C)=O)=O>>C(=O)(OC(C)(C)C)N[C@@H](C(C)C)C(=O)OCCCC(=O)O
c1ccc(C[O:21][C:19]([CH2:18][CH2:17][CH2:16][O:15][C:13]([C@H:4]([CH:2]([CH3:1])[CH3:3])[NH:5][C:6](=[O:7])[O:8][C:9]([CH3:10])([CH3:11])[CH3:12])=[O:14])=[O:20])cc1>>[CH3:1][CH:2]([CH3:3])[C@H:4]([NH:5][C:6](=[O:7])[O:8][C:9]([CH3:10])([CH3:11])[CH3:12])[C:13](=[O:14])[O:15][CH2:16][CH2:17][CH2:18][C:19](=[O:20])[OH:2...
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCCCC(=O)OCc1ccccc1
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCCCC(=O)O
null
[Pd]
C(C)(=O)OCC.CO
Deprotection
Ester saponification (alkyl deprotection)
86a971d3e4f88009ab4c98512e9f1deb51b2f0ce5cbd068cc61ae878c1e58e2a
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
null
[C:1]-[C:2](=[O;D1;H0:3])-[O;H0;D2;+0:4]-C-c1:c:c:c:c:c:1>>[C:1]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:4]
null
[]
null
null
2
HOUR
To a solution of 4-(N-Boc-L-valyloxy)butyric acid benzyl ester (1.2 g, 3 mmole) in ethyl acetate/methanol (5 ml/5 ml) was added palladium black (20 mg). The reaction mixture was kept under hydrogen at atmospheric pressure for 2 hr. The suspension was filtered through Celite and dried, giving the title product, 840 mg. ...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
c1ccccc1
null
null
Other
[Pd].C(C)(=O)OCC.CO
null
2
CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCCCC(=O)OCc1ccccc1>[Pd].C(C)(=O)OCC.CO>CC(C)[C@H](NC(=O)OC(C)(C)C)C(=O)OCCCC(=O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-215cdc25fad843078f46ce018c15b5cb
CC(C)(O)C(=O)O.COc1ccc(CCl)cc1>>COc1ccc(COC(=O)C(C)(C)O)cc1
C(C)O.OC(C(=O)O)(C)C.COC1=CC=C(CCl)C=C1>>OC(C(=O)OCC1=CC=C(C=C1)OC)(C)C
[OH:8][C:9](=[O:10])[C:11]([CH3:12])([CH3:13])[OH:14].Cl[CH2:7][c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:16][cH:15]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][O:8][C:9](=[O:10])[C:11]([CH3:12])([CH3:13])[OH:14])[cH:15][cH:16]1
CC(C)(O)C(=O)O.COc1ccc(CCl)cc1
COc1ccc(COC(=O)C(C)(C)O)cc1
null
null
ClCCl
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
06c4f868ad4646eea8208ecb83f54ca035dd62d04f0d8101641a4f487f2c695c
8446834f0edd1e71a2dcaffc09b80c7367abf3407263a8998354a2d20c1766bb
c1ccccc1
Cl-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[C:5]-[C:6](=[O;D1;H0:7])-[OH;D1;+0:8]>>[C:5]-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
2-hydroxy isobutyric acid (1.56 g) was esterified by alkylation with 4-methoxybenzyl chloride by the method described in Example A-I-1, step a). The title compound (2.65 g) was obtained after silica gel column chromatography (0, 1, 2% ethanol in dichloromethane). Rf (2% MeOH/CHCl3) 0.45. Conditions: See reaction.notes....
10.6084/m9.figshare.5104873.v1
null
Primary halide.Carboxylic acid
Ester
null
null
c1ccccc1
HCl
ClCCl
null
null
CC(C)(O)C(=O)O.COc1ccc(CCl)cc1>ClCCl>COc1ccc(COC(=O)C(C)(C)O)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-cd103c8f4bed475198a3058a6dfc2bc0
CC(C)[C@H](O)C(=O)O.COc1ccc(CCl)cc1>>COc1ccc(COC(=O)[C@@H](O)C(C)C)cc1
C(C)O.O[C@H](C(=O)O)C(C)C.COC1=CC=C(CCl)C=C1>>O[C@H](C(=O)OCC1=CC=C(C=C1)OC)C(C)C
[OH:8][C:9](=[O:10])[C@@H:11]([OH:12])[CH:13]([CH3:14])[CH3:15].Cl[CH2:7][c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:17][cH:16]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][O:8][C:9](=[O:10])[C@@H:11]([OH:12])[CH:13]([CH3:14])[CH3:15])[cH:16][cH:17]1
CC(C)[C@H](O)C(=O)O.COc1ccc(CCl)cc1
COc1ccc(COC(=O)[C@@H](O)C(C)C)cc1
null
null
ClCCl
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
06c4f868ad4646eea8208ecb83f54ca035dd62d04f0d8101641a4f487f2c695c
8446834f0edd1e71a2dcaffc09b80c7367abf3407263a8998354a2d20c1766bb
c1ccccc1
Cl-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[C:5]-[C:6](=[O;D1;H0:7])-[OH;D1;+0:8]>>[C:5]-[C:6](=[O;D1;H0:7])-[O;H0;D2;+0:8]-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
2-hydroxy-3-methyl-(S)-(+)-butyric acid (1.77 g) was esterified by alkylation with 4-methoxybenzyl chloride by the method described in Example A-I-1, step a. The title compound (3.10 g) was obtained after silica gel column chromatography (0, 1, 2% ethanol in dichloromethane). Rf (2% MeOH/CHCl3) 0.50. Conditions: See re...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Carboxylic acid
Ester
null
null
c1ccccc1
HCl
ClCCl
null
null
CC(C)[C@H](O)C(=O)O.COc1ccc(CCl)cc1>ClCCl>COc1ccc(COC(=O)[C@@H](O)C(C)C)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d1f715994313416e96876e3bf88df36c
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)O.COc1ccc(COC(=O)[C@@H](O)C(C)C)cc1>>COc1ccc(COC(=O)[C@@H](OC(=O)[C@@H](NC(=O)OCc2ccccc2)C(C)C)C(C)C)cc1
C(C)O.O[C@H](C(=O)OCC1=CC=C(C=C1)OC)C(C)C.C(C1=CC=CC=C1)OC(=O)N[C@@H](C(C)C)C(=O)O>>C(C1=CC=CC=C1)OC(=O)N[C@@H](C(C)C)C(=O)O[C@H](C(=O)OCC1=CC=C(C=C1)OC)C(C)C
O[C:13](=[O:14])[C@@H:15]([NH:16][C:17](=[O:18])[O:19][CH2:20][c:21]1[cH:22][cH:23][cH:24][cH:25][cH:26]1)[CH:27]([CH3:28])[CH3:29].[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][O:8][C:9](=[O:10])[C@@H:11]([OH:12])[CH:30]([CH3:31])[CH3:32])[cH:33][cH:34]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][O:8][C:9](=[O:10])[C@...
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)O.COc1ccc(COC(=O)[C@@H](O)C(C)C)cc1
COc1ccc(COC(=O)[C@@H](OC(=O)[C@@H](NC(=O)OCc2ccccc2)C(C)C)C(C)C)cc1
null
null
ClCCl
Acylation
Esterification of Carboxylic Acids
e916c5b009194e30c618975b40d7a233bfcf81339e65494c4e365f67cc5e011d
12ba7405a548c6b1674f05065819c74f53f1b6165cd54e84e1f2f208042fe660
O=C(CNC(=O)OCc1ccccc1)OCC(=O)OCc1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[#7:5]-[C:6]=[O;D1;H0:7].[C:8]-[C:9](-[OH;D1;+0:10])-[C:11](=[O;D1;H0:12])-[#8:13]-[C:14]>>[C:4]-[C:3](-[#7:5]-[C:6]=[O;D1;H0:7])-[C;H0;D3;+0:1](=[O;D1;H0:2])-[O;H0;D2;+0:10]-[C:9](-[C:8])-[C:11](=[O;D1;H0:12])-[#8:13]-[C:14]
null
[]
null
null
null
null
4-Methoxybenzyl 2-hydroxy-3-methyl-(S)-(+)-butyrate was acylated with N-benzyloxycarbonyl-L-valine by the method described in Example A-I-1, step b. The title compound (5.74 g) was obtained after silica gel column chromatography (0, 1, 1.5% ethanol in dichloromethane). Rf (2% MeOH/CHCl3) 0.70. Conditions: See reaction....
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary alcohol
Ester
null
null
c1ccccc1.c1ccccc1
HO-
ClCCl
null
null
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)O.COc1ccc(COC(=O)[C@@H](O)C(C)C)cc1>ClCCl>COc1ccc(COC(=O)[C@@H](OC(=O)[C@@H](NC(=O)OCc2ccccc2)C(C)C)C(C)C)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-acbc843521ff4b1886d8f94e72a0578d
COc1ccc(COC(=O)[C@@H](OC(=O)[C@@H](NC(=O)OCc2ccccc2)C(C)C)C(C)C)cc1>>CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)O[C@H](C(=O)O)C(C)C
C(C)O.C(C1=CC=CC=C1)OC(=O)N[C@@H](C(C)C)C(=O)O[C@H](C(=O)OCC1=CC=C(C=C1)OC)C(C)C>>C(C1=CC=CC=C1)OC(=O)N[C@@H](C(C)C)C(=O)O[C@H](C(=O)O)C(C)C
COc1ccc(C[O:22][C:20]([C@@H:19]([O:18][C:16]([C@H:4]([CH:2]([CH3:1])[CH3:3])[NH:5][C:6](=[O:7])[O:8][CH2:9][c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)=[O:17])[CH:23]([CH3:24])[CH3:25])=[O:21])cc1>>[CH3:1][CH:2]([CH3:3])[C@H:4]([NH:5][C:6](=[O:7])[O:8][CH2:9][c:10]1[cH:11][cH:12][cH:13][cH:14][cH:15]1)[C:16](=[O:17])[O...
COc1ccc(COC(=O)[C@@H](OC(=O)[C@@H](NC(=O)OCc2ccccc2)C(C)C)C(C)C)cc1
CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)O[C@H](C(=O)O)C(C)C
null
null
ClCCl
Reduction
Ester saponification (alkyl deprotection)
af4a00273af84ecb3074b1842201a78a3aac9a41d2050132ad8c8c1c9d796dee
8d997f8b7994d8c9cf23425771b3f80d4d4830ac4e3d6552f381db244a5a65c5
c1ccccc1
C-O-c1:c:c:c(-C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]):c:c:1>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
null
[]
null
null
null
null
4-methoxybenzyl 2-(N-benzyloxycarbonyl-L-valyloxy)-3-methyl-(S)-(+)-butyrate was de-esterified by the method described in Example A-I-1, step c. The title compound (3.41 g) was obtained after silica gel column chromatography (2, 10, 20% ethanol in dichloromethane). Rf (2% MeOH/CHCl3) 0.45. The compound may be activated...
10.6084/m9.figshare.5104873.v1
null
Ester.Ether
Carboxylic acid
c1ccccc1
null
c1ccccc1
HO-
ClCCl
null
null
COc1ccc(COC(=O)[C@@H](OC(=O)[C@@H](NC(=O)OCc2ccccc2)C(C)C)C(C)C)cc1>ClCCl>CC(C)[C@H](NC(=O)OCc1ccccc1)C(=O)O[C@H](C(=O)O)C(C)C