dataset_id
large_stringclasses
414 values
reaction_id
large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
reactant_smiles
large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0f218942ee1f4928a90ada5177e921b7
NCc1ccccc1.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1>>O=C1Cc2cc(S(=O)(=O)NCc3ccccc3)ccc2N1
Cl.ClS(=O)(=O)C=1C=C2CC(NC2=CC1)=O.C(C1=CC=CC=C1)N.N1=CC=CC=C1>>C(C1=CC=CC=C1)NS(=O)(=O)C=1C=C2CC(NC2=CC1)=O
[NH2:10][CH2:11][c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1.Cl[S:7]([c:6]1[cH:5][c:4]2[c:20]([cH:19][cH:18]1)[NH:21][C:2](=[O:1])[CH2:3]2)(=[O:8])=[O:9]>>[O:1]=[C:2]1[CH2:3][c:4]2[cH:5][c:6]([S:7](=[O:8])(=[O:9])[NH:10][CH2:11][c:12]3[cH:13][cH:14][cH:15][cH:16][cH:17]3)[cH:18][cH:19][c:20]2[NH:21]1
NCc1ccccc1.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1
O=C1Cc2cc(S(=O)(=O)NCc3ccccc3)ccc2N1
null
null
ClCCl.C(C)(=O)OCC
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=C1Cc2cc(S(=O)(=O)NCc3ccccc3)ccc2N1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[NH2;D1;+0:7]-[C:8]-[c:9]>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[NH;D2;+0:7]-[C:8]-[c:9])-[c:4](:[c:5]):[c:6]
66.1
[{"value": 66.0, "product": "C(C1=CC=CC=C1)NS(=O)(=O)C=1C=C2CC(NC2=CC1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 66.1, "product": "C(C1=CC=CC=C1)NS(=O)(=O)C=1C=C2CC(NC2=CC1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
A suspension of 5-chlorosulfonyl-2-oxindole (1.62 g, 7 mmol), benzylamine (0.918 mL, 8.4 mmol) and pyridine (1 mL) in dichloromethane (20 mL) was stirred at room temperature for 4 hours. The reaction mixture was diluted with ethyl acetate (300 mL) and acidified with 1 N hydrochloric acid (16 mL). The organic layer was ...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccc2c(c1)CCN2.c1ccccc1
HCl
ClCCl.C(C)(=O)OCC
null
4
NCc1ccccc1.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1>ClCCl.C(C)(=O)OCC>O=C1Cc2cc(S(=O)(=O)NCc3ccccc3)ccc2N1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b80eeb8993cb48e39afe93a6e754ca1a
NCc1ccc(F)cc1.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1>>O=C1Cc2cc(S(=O)(=O)NCc3ccc(F)cc3)ccc2N1
ClS(=O)(=O)C=1C=C2CC(NC2=CC1)=O.FC1=CC=C(CN)C=C1.N1=CC=CC=C1>>FC1=CC=C(CNS(=O)(=O)C=2C=C3CC(NC3=CC2)=O)C=C1
[NH2:10][CH2:11][c:12]1[cH:13][cH:14][c:15]([F:16])[cH:17][cH:18]1.Cl[S:7]([c:6]1[cH:5][c:4]2[c:21]([cH:20][cH:19]1)[NH:22][C:2](=[O:1])[CH2:3]2)(=[O:8])=[O:9]>>[O:1]=[C:2]1[CH2:3][c:4]2[cH:5][c:6]([S:7](=[O:8])(=[O:9])[NH:10][CH2:11][c:12]3[cH:13][cH:14][c:15]([F:16])[cH:17][cH:18]3)[cH:19][cH:20][c:21]2[NH:22]1
NCc1ccc(F)cc1.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1
O=C1Cc2cc(S(=O)(=O)NCc3ccc(F)cc3)ccc2N1
null
null
ClCCl
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=C1Cc2cc(S(=O)(=O)NCc3ccccc3)ccc2N1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[NH2;D1;+0:7]-[C:8]-[c:9]>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[NH;D2;+0:7]-[C:8]-[c:9])-[c:4](:[c:5]):[c:6]
84
[{"value": 84.0, "product": "FC1=CC=C(CNS(=O)(=O)C=2C=C3CC(NC3=CC2)=O)C=C1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
A suspension of 5-chlorosulfonyl-2-oxindole (5.0 g), 4-fluorobenzylamine (3.0 mL) and pyridine (3.5 mL) in dichloromethane (30 mL) was stirred at room temperature for 4 hours. The precipitate was filtered, washed with dichloromethane and dried to give 5.8 g (84%) of 2-oxo-2,3-dihydro-1H-indole-5-sulfonic acid 4-fluoro-...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccc2c(c1)CCN2.c1ccccc1
HCl
ClCCl
null
4
NCc1ccc(F)cc1.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1>ClCCl>O=C1Cc2cc(S(=O)(=O)NCc3ccc(F)cc3)ccc2N1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-9512e5995e1e4f05808eeea03d9e3e61
Nc1cccc(Cl)c1.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1>>O=C1Cc2cc(S(=O)(=O)Nc3cccc(Cl)c3)ccc2N1
ClS(=O)(=O)C=1C=C2CC(NC2=CC1)=O.ClC=1C=C(N)C=CC1.N1=CC=CC=C1>>ClC=1C=C(C=CC1)NS(=O)(=O)C=1C=C2CC(NC2=CC1)=O
[NH2:10][c:11]1[cH:12][cH:13][cH:14][c:15]([Cl:16])[cH:17]1.Cl[S:7]([c:6]1[cH:5][c:4]2[c:20]([cH:19][cH:18]1)[NH:21][C:2](=[O:1])[CH2:3]2)(=[O:8])=[O:9]>>[O:1]=[C:2]1[CH2:3][c:4]2[cH:5][c:6]([S:7](=[O:8])(=[O:9])[NH:10][c:11]3[cH:12][cH:13][cH:14][c:15]([Cl:16])[cH:17]3)[cH:18][cH:19][c:20]2[NH:21]1
Nc1cccc(Cl)c1.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1
O=C1Cc2cc(S(=O)(=O)Nc3cccc(Cl)c3)ccc2N1
null
null
ClCCl
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=C1Cc2cc(S(=O)(=O)Nc3ccccc3)ccc2N1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[NH2;D1;+0:7]-[c:8](:[c:9]):[c:10]>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[NH;D2;+0:7]-[c:8](:[c:9]):[c:10])-[c:4](:[c:5]):[c:6]
74
[{"value": 74.0, "product": "ClC=1C=C(C=CC1)NS(=O)(=O)C=1C=C2CC(NC2=CC1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
A suspension of 5-chlorosulfonyl-2-oxindole (5 g), 3-chloroaniline (2.74 mL) and pyridine (3.5 mL) in dichloromethane (30 mL) was stirred at room temperature for overnight. The precipitate was filtered, washed with dichloromethane and dried to give 5.2 g (74%) 2-oxo-2,3-dihydro-1H-indole-5-sulfonic acid (3-chloro-pheny...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccc2c(c1)CCN2.c1ccccc1
HCl
ClCCl
null
8
Nc1cccc(Cl)c1.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1>ClCCl>O=C1Cc2cc(S(=O)(=O)Nc3cccc(Cl)c3)ccc2N1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b71dcc59c17f45b0a42c35086404e79c
COc1ccccc1N.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1>>COc1ccccc1NS(=O)(=O)c1ccc2c(c1)CC(=O)N2
ClS(=O)(=O)C=1C=C2CC(NC2=CC1)=O.COC=1C(=CC=CC1)N.N1=CC=CC=C1>>COC1=C(C=CC=C1)NS(=O)(=O)C=1C=C2CC(NC2=CC1)=O
[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][cH:7][c:8]1[NH2:9].Cl[S:10](=[O:11])(=[O:12])[c:13]1[cH:14][cH:15][c:16]2[c:17]([cH:18]1)[CH2:19][C:20](=[O:21])[NH:22]2>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][cH:7][c:8]1[NH:9][S:10](=[O:11])(=[O:12])[c:13]1[cH:14][cH:15][c:16]2[c:17]([cH:18]1)[CH2:19][C:20](=[O:21])[NH:22]2
COc1ccccc1N.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1
COc1ccccc1NS(=O)(=O)c1ccc2c(c1)CC(=O)N2
null
null
ClCCl
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=C1Cc2cc(S(=O)(=O)Nc3ccccc3)ccc2N1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[NH2;D1;+0:7]-[c:8](:[c:9]):[c:10]>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[NH;D2;+0:7]-[c:8](:[c:9]):[c:10])-[c:4](:[c:5]):[c:6]
37
[{"value": 37.0, "product": "COC1=C(C=CC=C1)NS(=O)(=O)C=1C=C2CC(NC2=CC1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 5-chlorosulfonyl-2-oxindole (3 g), o-anisidine (1.8 mL) and pyridine (2.1 mL) in dichloromethane (20 mL) was stirred at room temperature for overnight at which time the red color solid was present. The solid was filtered, washed with ethanol and dried under vacuum to yield 1.5 g (37%) of 2-oxo-2,3-dihydro...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccccc1.c1ccc2c(c1)CCN2
HCl
ClCCl
null
null
COc1ccccc1N.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1>ClCCl>COc1ccccc1NS(=O)(=O)c1ccc2c(c1)CC(=O)N2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-49d25400c31f48409a84e78483e89006
Nc1cccnc1.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1>>O=C1Cc2cc(S(=O)(=O)Nc3cccnc3)ccc2N1
ClS(=O)(=O)C=1C=C2CC(NC2=CC1)=O.NC=1C=NC=CC1>>N1=CC(=CC=C1)NS(=O)(=O)C=1C=C2CC(NC2=CC1)=O
[NH2:10][c:11]1[cH:12][cH:13][cH:14][n:15][cH:16]1.Cl[S:7]([c:6]1[cH:5][c:4]2[c:19]([cH:18][cH:17]1)[NH:20][C:2](=[O:1])[CH2:3]2)(=[O:8])=[O:9]>>[O:1]=[C:2]1[CH2:3][c:4]2[cH:5][c:6]([S:7](=[O:8])(=[O:9])[NH:10][c:11]3[cH:12][cH:13][cH:14][n:15][cH:16]3)[cH:17][cH:18][c:19]2[NH:20]1
Nc1cccnc1.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1
O=C1Cc2cc(S(=O)(=O)Nc3cccnc3)ccc2N1
null
null
N1=CC=CC=C1
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=C1Cc2cc(S(=O)(=O)Nc3cccnc3)ccc2N1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[NH2;D1;+0:7]-[c:8](:[c:9]):[c:10]:[#7;a:11]:[c:12]>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[NH;D2;+0:7]-[c:8](:[c:9]):[c:10]:[#7;a:11]:[c:12])-[c:4](:[c:5]):[c:6]
38
[{"value": 38.0, "product": "N1=CC(=CC=C1)NS(=O)(=O)C=1C=C2CC(NC2=CC1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 37.4, "product": "N1=CC(=CC=C1)NS(=O)(=O)C=1C=C2CC(NC2=CC1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 5-chlorosulfonyl-2-oxindole (3 g) and 3-aminopyridine (1.46 g) in pyridine (15 mL) was stirred at room temperature for overnight at which time the brown color solid was present. The precipitate was filtered, washed with ethanol and dried under vacuum to yield 1.4 g (38%) of 2-oxo-2,3-dihydro-1H-indole-5-s...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccc2c(c1)CCN2.c1ccncc1
HCl
N1=CC=CC=C1
null
null
Nc1cccnc1.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1>N1=CC=CC=C1>O=C1Cc2cc(S(=O)(=O)Nc3cccnc3)ccc2N1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-761f226795de4ac6b0c3118f5cfe2d33
COCCN.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1>>COCCNS(=O)(=O)c1ccc2c(c1)CC(=O)N2
ClS(=O)(=O)C=1C=C2CC(NC2=CC1)=O.COCCN.N1=CC=CC=C1>>COCCNS(=O)(=O)C=1C=C2CC(NC2=CC1)=O
[CH3:1][O:2][CH2:3][CH2:4][NH2:5].Cl[S:6](=[O:7])(=[O:8])[c:9]1[cH:10][cH:11][c:12]2[c:13]([cH:14]1)[CH2:15][C:16](=[O:17])[NH:18]2>>[CH3:1][O:2][CH2:3][CH2:4][NH:5][S:6](=[O:7])(=[O:8])[c:9]1[cH:10][cH:11][c:12]2[c:13]([cH:14]1)[CH2:15][C:16](=[O:17])[NH:18]2
COCCN.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1
COCCNS(=O)(=O)c1ccc2c(c1)CC(=O)N2
null
null
ClCCl
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=C1Cc2ccccc2N1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[C:7]-[C:8]-[NH2;D1;+0:9]>>[C:7]-[C:8]-[NH;D2;+0:9]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]
33
[{"value": 33.0, "product": "COCCNS(=O)(=O)C=1C=C2CC(NC2=CC1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 5-chlorosulfonyl-2-oxindole (5 g), 2-methoxyethylamine (2.25 mL) and pyridine (7 mL) in dichloromethane (30 mL) was stirred at room temperature for 4 hours. The reaction was concentrated and dichloromethane (15 mL) was added. The precipitate was filtered, washed with dichloromethane and dried to give 1.9 ...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccc2c(c1)CCN2
HCl
ClCCl
null
null
COCCN.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1>ClCCl>COCCNS(=O)(=O)c1ccc2c(c1)CC(=O)N2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4fe8631dc68e4b4fafdf204b79c372cd
O=C1Cc2ccccc2N1.O=S(=O)(O)Cl>>O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1
ClS(=O)(=O)O.N1C(CC2=CC=CC=C12)=O>>ClS(=O)(=O)C=1C=C2CC(NC2=CC1)=O
[O:1]=[C:2]1[CH2:3][c:4]2[cH:5][cH:6][cH:11][cH:12][c:13]2[NH:14]1.O[S:7](=[O:8])(=[O:9])[Cl:10]>>[O:1]=[C:2]1[CH2:3][c:4]2[cH:5][c:6]([S:7](=[O:8])(=[O:9])[Cl:10])[cH:11][cH:12][c:13]2[NH:14]1
O=C1Cc2ccccc2N1.O=S(=O)(O)Cl
O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1
null
null
O
Heteroatom Alkylation and Arylation
Aromatic sulfonyl chlorination
1d9d5a8f3073ec09a40a230cbc17ee68db12527a82342f5e24b541bcc0969ba1
d32b60b8f9bfd187c6c9f1eef6a22a00f53525a7532b83aba763d5389c9e4280
O=C1Cc2ccccc2N1
O-[S;H0;D4;+0:1](-[Cl;D1;H0:2])(=[O;D1;H0:3])=[O;D1;H0:4].[c:5]:[c:6]:[cH;D2;+0:7]:[c:8]:[c:9]>>[Cl;D1;H0:2]-[S;H0;D4;+0:1](=[O;D1;H0:3])(=[O;D1;H0:4])-[c;H0;D3;+0:7](:[c:6]:[c:5]):[c:8]:[c:9]
50
[{"value": 50.0, "product": "ClS(=O)(=O)C=1C=C2CC(NC2=CC1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
1.5
HOUR
To a 100 mL flask charged with 27 mL of chlorosulfonic acid, 13.3 g of 2-oxindole was added slowly. The reaction temperature was maintained below 30° C. during the addition. After the addition, the reaction mixture was stirred at room temperature for 1.5 hour, heated to 68° C. for 1 hour, cooled, and poured into water....
10.6084/m9.figshare.5104873.v1
null
null
Sulfonyl halide
c1ccc2c(c1)CCN2
c1ccc2c(c1)CCN2
c1ccc2c(c1)CCN2
HO-
O
null
1.5
O=C1Cc2ccccc2N1.O=S(=O)(O)Cl>O>O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b820d9b2cbf24448ad491e3ac1473356
O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1.[NH4+]>>NS(=O)(=O)c1ccc2c(c1)CC(=O)N2
ClS(=O)(=O)C=1C=C2CC(NC2=CC1)=O.[OH-].[NH4+]>>NS(=O)(=O)C=1C=C2CC(NC2=CC1)=O
Cl[S:2](=[O:3])(=[O:4])[c:5]1[cH:6][cH:7][c:8]2[c:9]([cH:10]1)[CH2:11][C:12](=[O:13])[NH:14]2.[NH4+:1]>>[NH2:1][S:2](=[O:3])(=[O:4])[c:5]1[cH:6][cH:7][c:8]2[c:9]([cH:10]1)[CH2:11][C:12](=[O:13])[NH:14]2
O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1.[NH4+]
NS(=O)(=O)c1ccc2c(c1)CC(=O)N2
null
null
C(C)O
Acylation
OtherReaction
672a14b4f1ef0b966898e1b4c118f241f21df1d6e087372155b9d0c840dac61f
29e1633db8f1f00444181a0bcac91d574ed806fddf9165be4c8478fc32a80994
O=C1Cc2ccccc2N1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[NH4+;D0:7]>>[NH2;D1;+0:7]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]
20
[{"value": 20.0, "product": "NS(=O)(=O)C=1C=C2CC(NC2=CC1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
5-Chlorosulfonyl-2-oxindole (2.1 g) was added to 10 mL of ammonium hydroxide in 10 mL of ethanol and stirred at room temperature overnight. The mixture was concentrated and the solid collected by vacuum filtration to give 0.4 g (20% yield) of 5-aminosulfonyl-2-oxindole as an off-white solid. Conditions: See reaction.no...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
Sulfonamide
null
null
c1ccc2c(c1)CCN2
HCl
C(C)O
null
8
O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1.[NH4+]>C(C)O>NS(=O)(=O)c1ccc2c(c1)CC(=O)N2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-cc2860086c3648638a6b6a5ca5490ccd
CN.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1>>CNS(=O)(=O)c1ccc2c(c1)CC(=O)N2
ClS(=O)(=O)C=1C=C2CC(NC2=CC1)=O.CN>>CNS(=O)(=O)C=1C=C2CC(NC2=CC1)=O
[CH3:1][NH2:2].Cl[S:3](=[O:4])(=[O:5])[c:6]1[cH:7][cH:8][c:9]2[c:10]([cH:11]1)[CH2:12][C:13](=[O:14])[NH:15]2>>[CH3:1][NH:2][S:3](=[O:4])(=[O:5])[c:6]1[cH:7][cH:8][c:9]2[c:10]([cH:11]1)[CH2:12][C:13](=[O:14])[NH:15]2
CN.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1
CNS(=O)(=O)c1ccc2c(c1)CC(=O)N2
null
null
O1CCCC1
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=C1Cc2ccccc2N1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[C;D1;H3:7]-[NH2;D1;+0:8]>>[C;D1;H3:7]-[NH;D2;+0:8]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]
88
[{"value": 88.0, "product": "CNS(=O)(=O)C=1C=C2CC(NC2=CC1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
A suspension of 3.38 g of 5-chlorosulfonyl-2-oxindole in 10 mL of 2 M methylamine in tetrahydrofuran was stirred at room temperature for 4 hours at which time a white solid was present. The precipitate was collected by vacuum filtration, washed twice with 5 mL of water each time and dried under vacuum at 40° C. overnig...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccc2c(c1)CCN2
HCl
O1CCCC1
null
4
CN.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1>O1CCCC1>CNS(=O)(=O)c1ccc2c(c1)CC(=O)N2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c04674d1561d4ba9821fdd21961b06c9
CNC.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1>>CN(C)S(=O)(=O)c1ccc2c(c1)CC(=O)N2
ClS(=O)(=O)C=1C=C2CC(NC2=CC1)=O.CNC>>CN(S(=O)(=O)C=1C=C2CC(NC2=CC1)=O)C
[CH3:1][NH:2][CH3:3].Cl[S:4](=[O:5])(=[O:6])[c:7]1[cH:8][cH:9][c:10]2[c:11]([cH:12]1)[CH2:13][C:14](=[O:15])[NH:16]2>>[CH3:1][N:2]([CH3:3])[S:4](=[O:5])(=[O:6])[c:7]1[cH:8][cH:9][c:10]2[c:11]([cH:12]1)[CH2:13][C:14](=[O:15])[NH:16]2
CNC.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1
CN(C)S(=O)(=O)c1ccc2c(c1)CC(=O)N2
null
null
CO
Acylation
Sulfonamide synthesis (Schotten-Baumann) secondary amine
abeb6d9a0c70fe5baef0a8e555c2cd55ac2317f763ce7a0831775db7a04777d8
b7aca5a5d690b0846685a854bc946849e1041bfc3965161290b5ffb2821af09e
O=C1Cc2ccccc2N1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[C;D1;H3:7]-[NH;D2;+0:8]-[C;D1;H3:9]>>[C;D1;H3:7]-[N;H0;D3;+0:8](-[C;D1;H3:9])-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]
79
[{"value": 79.0, "product": "CN(S(=O)(=O)C=1C=C2CC(NC2=CC1)=O)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
A suspension of 2.3 g of 5-chlorosulfonyl-2-oxindole in 10 mL of 2 M dimethylamine in methanol was stirred at room temperature for 4 hours at which time a white solid was present. The precipitate was collected by vacuum filtration, washed with 5 mL of 1 N sodium hydroxide and 5 mL of 1 N hydrochloric acid and dried und...
10.6084/m9.figshare.5104873.v1
null
Secondary amine.Sulfonyl halide
Tertiary amine
null
null
c1ccc2c(c1)CCN2
HCl
CO
null
4
CNC.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1>CO>CN(C)S(=O)(=O)c1ccc2c(c1)CC(=O)N2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-8db5f9b6624f4568a95dc50f93c1c1cd
CC(C)N.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1>>CC(C)NS(=O)(=O)c1ccc2c(c1)CC(=O)N2
ClS(=O)(=O)C=1C=C2CC(NC2=CC1)=O.C(C)(C)N.N1=CC=CC=C1>>C(C)(C)NS(=O)(=O)C=1C=C2CC(NC2=CC1)=O
[CH3:1][CH:2]([CH3:3])[NH2:4].Cl[S:5](=[O:6])(=[O:7])[c:8]1[cH:9][cH:10][c:11]2[c:12]([cH:13]1)[CH2:14][C:15](=[O:16])[NH:17]2>>[CH3:1][CH:2]([CH3:3])[NH:4][S:5](=[O:6])(=[O:7])[c:8]1[cH:9][cH:10][c:11]2[c:12]([cH:13]1)[CH2:14][C:15](=[O:16])[NH:17]2
CC(C)N.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1
CC(C)NS(=O)(=O)c1ccc2c(c1)CC(=O)N2
null
null
ClCCl
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=C1Cc2ccccc2N1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[C;D1;H3:7]-[C:8](-[C;D1;H3:9])-[NH2;D1;+0:10]>>[C;D1;H3:7]-[C:8](-[C;D1;H3:9])-[NH;D2;+0:10]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]
45.5
[{"value": 45.0, "product": "C(C)(C)NS(=O)(=O)C=1C=C2CC(NC2=CC1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 45.5, "product": "C(C)(C)NS(=O)(=O)C=1C=C2CC(NC2=CC1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
A suspension of 3 g of 5-chlorosulfonyl-2-oxindole, 1.15 g of isopropylamine and 1.2 mL of pyridine in 50 mL of dichloromethane was stirred at room temperature for 4 hours at which time a white solid was present. The precipitate was collected by vacuum filtration. The solids were slurry-washed with hot ethanol, cooled,...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccc2c(c1)CCN2
HCl
ClCCl
null
4
CC(C)N.O=C1Cc2cc(S(=O)(=O)Cl)ccc2N1>ClCCl>CC(C)NS(=O)(=O)c1ccc2c(c1)CC(=O)N2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a8fff4cc818e435b81ea9979252c47a9
O=C1Cc2cc(Br)ccc2N1.OB(O)c1ccccc1>>O=C1Cc2cc(-c3ccccc3)ccc2N1
C1(=CC=CC=C1)B(O)O.C([O-])([O-])=O.[Na+].[Na+].BrC=1C=C2CC(NC2=CC1)=O.C(C)O>>C1(=CC=CC=C1)C=1C=C2CC(NC2=CC1)=O
Br[c:6]1[cH:5][c:4]2[c:15]([cH:14][cH:13]1)[NH:16][C:2](=[O:1])[CH2:3]2.OB(O)[c:7]1[cH:8][cH:9][cH:10][cH:11][cH:12]1>>[O:1]=[C:2]1[CH2:3][c:4]2[cH:5][c:6](-[c:7]3[cH:8][cH:9][cH:10][cH:11][cH:12]3)[cH:13][cH:14][c:15]2[NH:16]1
O=C1Cc2cc(Br)ccc2N1.OB(O)c1ccccc1
O=C1Cc2cc(-c3ccccc3)ccc2N1
null
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1
C1(=CC=CC=C1)C.C(C)(=O)OCC
C-C Coupling
Suzuki coupling with boronic acids
9791290dea007c134587598bd16674eb122eb7281e427c61b6d8f55d72a5f584
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Cc2cc(-c3ccccc3)ccc2N1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:8]:[c:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9]:[c:10]
77.3
[{"value": 77.0, "product": "C1(=CC=CC=C1)C=1C=C2CC(NC2=CC1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 77.3, "product": "C1(=CC=CC=C1)C=1C=C2CC(NC2=CC1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
12
HOUR
5-Bromo-2-oxindole (5 g, 23.5 mmol) was dissolved in 110 mL of toluene and 110 mL of ethanol with stirring and a little heating. Tetrakis(triphenylphosphine)-palladium(0) (1.9 g, 1.6 mmol) was added followed by a 2 M aq. solution of sodium carbonate (40 mL, 80 mmol). To this mixture benzene boronic acid (3.7 g, 30.6 mm...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2c(c1)CCN2.c1ccccc1
c1ccc2c(c1)CCN2.c1ccccc1
c1ccc2c(c1)CCN2.c1ccccc1
HBr.B
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)C.C(C)(=O)OCC
100
12
O=C1Cc2cc(Br)ccc2N1.OB(O)c1ccccc1>[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)C.C(C)(=O)OCC>O=C1Cc2cc(-c3ccccc3)ccc2N1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5a35eb37090d4673953f933d414f1791
O=C1Cc2ccc(Br)cc2N1.OB(O)c1cccnc1>>O=C1Cc2ccc(-c3cccnc3)cc2N1
C([O-])([O-])=O.[Na+].[Na+].C(CC)(O)O.N1=CC(=CC=C1)B(O)O.C(C)O.BrC1=CC=C2CC(NC2=C1)=O>>N1=CC(=CC=C1)C1=CC=C2CC(NC2=C1)=O
Br[c:7]1[cH:6][cH:5][c:4]2[c:15]([cH:14]1)[NH:16][C:2](=[O:1])[CH2:3]2.OB(O)[c:8]1[cH:9][cH:10][cH:11][n:12][cH:13]1>>[O:1]=[C:2]1[CH2:3][c:4]2[cH:5][cH:6][c:7](-[c:8]3[cH:9][cH:10][cH:11][n:12][cH:13]3)[cH:14][c:15]2[NH:16]1
O=C1Cc2ccc(Br)cc2N1.OB(O)c1cccnc1
O=C1Cc2ccc(-c3cccnc3)cc2N1
null
null
C1(=CC=CC=C1)C.C(C)(=O)OCC
C-C Coupling
Suzuki coupling with boronic acids
a91ebef74c819bbf975cd59349af7e75fd7403a76d7a54fde0217a7e75825ae7
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Cc2ccc(-c3cccnc3)cc2N1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]-[#7:4]):[c:5]:[c:6].O-B(-O)-[c;H0;D3;+0:7]1:[c:8]:[#7;a:9]:[c:10]:[c:11]:[c:12]:1>>[#7:4]-[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:7]1:[c:8]:[#7;a:9]:[c:10]:[c:11]:[c:12]:1):[c:5]:[c:6]
42
[{"value": 42.0, "product": "N1=CC(=CC=C1)C1=CC=C2CC(NC2=C1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 42.0, "product": "N1=CC(=CC=C1)C1=CC=C2CC(NC2=C1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
null
null
To a solution of 6-bromo-2-oxindole (4 g, 26.3 mmol) dissolved in 60 mL of toluene and 60 mL of ethanol with stirring and a little heating tetrakis(triphenyl-phosphine)palladium(0) (2.3 g, 1.9 mmol) was added followed by a 2 M aqueous solution of sodium carbonate (50 mL, 100 mmol) and pyridine-3-boronic acid propane di...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2c(c1)CCN2.c1ccncc1
c1ccc2c(c1)CCN2.c1ccncc1
c1ccc2c(c1)CCN2.c1ccncc1
HBr.B
C1(=CC=CC=C1)C.C(C)(=O)OCC
100
null
O=C1Cc2ccc(Br)cc2N1.OB(O)c1cccnc1>C1(=CC=CC=C1)C.C(C)(=O)OCC>O=C1Cc2ccc(-c3cccnc3)cc2N1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-55ea1a3635b74f3a8ec5c8236a434314
O=[N+]([O-])c1cc(Br)ccc1F.OB(O)c1ccccc1>>O=[N+]([O-])c1cc(-c2ccccc2)ccc1F
C1(=CC=CC=C1)B(O)O.BrC=1C=CC(=C(C1)[N+](=O)[O-])F.C([O-])([O-])=O.[Na+].[Na+]>>FC1=C(C=C(C=C1)C1=CC=CC=C1)[N+](=O)[O-]
Br[c:6]1[cH:5][c:4]([N+:2](=[O:1])[O-:3])[c:15]([F:16])[cH:14][cH:13]1.OB(O)[c:7]1[cH:8][cH:9][cH:10][cH:11][cH:12]1>>[O:1]=[N+:2]([O-:3])[c:4]1[cH:5][c:6](-[c:7]2[cH:8][cH:9][cH:10][cH:11][cH:12]2)[cH:13][cH:14][c:15]1[F:16]
O=[N+]([O-])c1cc(Br)ccc1F.OB(O)c1ccccc1
O=[N+]([O-])c1cc(-c2ccccc2)ccc1F
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
C1(=CC=CC=C1)C.C(C)O
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccccc2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:8]:[c:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9]:[c:10]
96.2
[{"value": 96.0, "product": "FC1=C(C=C(C=C1)C1=CC=CC=C1)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 96.2, "product": "FC1=C(C=C(C=C1)C1=CC=CC=C1)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Tetrakis(triphenylphosphine)palladium (0.8 g) was added to a mixture of benzeneboronic acid (3.1 g), 5-bromo-2-fluoronitrobenzene (5 g) and 22 mL of 2 M sodium carbonate solution in toluene (50 mL) and ethanol (50 mL). The mixture was heated to reflux for 2 hours, concentrated, and the residue was extracted twice with ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C1(=CC=CC=C1)C.C(C)O
null
null
O=[N+]([O-])c1cc(Br)ccc1F.OB(O)c1ccccc1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C1(=CC=CC=C1)C.C(C)O>O=[N+]([O-])c1cc(-c2ccccc2)ccc1F
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-93f14a92d7b948aeb7136339faf59c3b
COC(=O)CC(=O)OC.O=[N+]([O-])c1cc(-c2ccccc2)ccc1F>>COC(=O)C(C(=O)OC)c1ccc(-c2ccccc2)cc1[N+](=O)[O-]
FC1=C(C=C(C=C1)C1=CC=CC=C1)[N+](=O)[O-].C(CC(=O)OC)(=O)OC.[H-].[Na+]>>COC(C(C(=O)OC)C1=C(C=C(C=C1)C1=CC=CC=C1)[N+](=O)[O-])=O
[CH3:1][O:2][C:3](=[O:4])[CH2:5][C:6](=[O:7])[O:8][CH3:9].F[c:10]1[cH:11][cH:12][c:13](-[c:14]2[cH:15][cH:16][cH:17][cH:18][cH:19]2)[cH:20][c:21]1[N+:22](=[O:23])[O-:24]>>[CH3:1][O:2][C:3](=[O:4])[CH:5]([C:6](=[O:7])[O:8][CH3:9])[c:10]1[cH:11][cH:12][c:13](-[c:14]2[cH:15][cH:16][cH:17][cH:18][cH:19]2)[cH:20][c:21]1[N+:...
COC(=O)CC(=O)OC.O=[N+]([O-])c1cc(-c2ccccc2)ccc1F
COC(=O)C(C(=O)OC)c1ccc(-c2ccccc2)cc1[N+](=O)[O-]
null
null
CS(=O)C
C-C Coupling
OtherReaction
5a1171068c2a10d196160f01101b1c97354196d6923cfc455c6b686284d6c6f2
c0fb657475d92a5e1ab643a3f03921ebe4d047c8d805f98b012a5df3f9fb1f6c
c1ccc(-c2ccccc2)cc1
F-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[#7;+:5]):[c:6].[C;D1;H3:7]-[#8:8]-[C:9](=[O;D1;H0:10])-[CH2;D2;+0:11]-[C:12](=[O;D1;H0:13])-[#8:14]-[C;D1;H3:15]>>[#7;+:5]-[c:4](:[c:6]):[c;H0;D3;+0:1](-[CH;D3;+0:11](-[C:9](=[O;D1;H0:10])-[#8:8]-[C;D1;H3:7])-[C:12](=[O;D1;H0:13])-[#8:14]-[C;D1;H3:15]):[c:2]:[c:3]
null
[]
100
CELSIUS
null
null
Dimethyl malonate (10 mL) in 25 mL of dimethylsulfoxide was added dropwise to 3.5 g of sodium hydride suspended in 25 mL of dimethylsulfoxide and the mixture heated at 100° C. for 10 minutes. The mixture was cooled to room temperature and 4.7 g of 4-fluoro-3-nitrobiphenyl in 25 mL of dimethylsulfoxide was added. The mi...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Ester
Ester.Ester
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1
HF
CS(=O)C
100
null
COC(=O)CC(=O)OC.O=[N+]([O-])c1cc(-c2ccccc2)ccc1F>CS(=O)C>COC(=O)C(C(=O)OC)c1ccc(-c2ccccc2)cc1[N+](=O)[O-]
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-72684266cfd64a47babebee184279430
O=C(O)Cc1ccc(-c2ccccc2)cc1[N+](=O)[O-]>>O=C1Cc2ccc(-c3ccccc3)cc2N1
[N+](=O)([O-])C=1C=C(C=CC1CC(=O)O)C1=CC=CC=C1>>C1(=CC=CC=C1)C1=CC=C2CC(NC2=C1)=O
O=[N+:16]([O-])[c:15]1[c:4]([CH2:3][C:2](O)=[O:1])[cH:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][cH:11][cH:12][cH:13]2)[cH:14]1>>[O:1]=[C:2]1[CH2:3][c:4]2[cH:5][cH:6][c:7](-[c:8]3[cH:9][cH:10][cH:11][cH:12][cH:13]3)[cH:14][c:15]2[NH:16]1
O=C(O)Cc1ccc(-c2ccccc2)cc1[N+](=O)[O-]
O=C1Cc2ccc(-c3ccccc3)cc2N1
null
[Fe]
C(C)(=O)O
Functional Group Interconversion
OtherReaction
e98c7e13a0e22318df8d26b28a8117bfb6ce0313bb5b14de92a87461040b8923
98c112fcc8dd821704dc378798368c2081a2acc574356674c70af3e59954ee0d
O=C1Cc2ccc(-c3ccccc3)cc2N1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[c:4]:[c:5](-[N+;H0;D3:6](=O)-[O-]):[c:7]>>[O;D1;H0:2]=[C;H0;D3;+0:1]1-[C:3]-[c:4]:[c:5](:[c:7])-[NH;D2;+0:6]-1
93
[{"value": 93.0, "product": "C1(=CC=CC=C1)C1=CC=C2CC(NC2=C1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 92.9, "product": "C1(=CC=CC=C1)C1=CC=C2CC(NC2=C1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Iron chips (2.6 g) were added all at once to 4.5 g of 3-nitrobiphenyl-4-acetic acid in 40 mL of acetic acid. The mixture was heated to reflux for 2 hours, concentrated to dryness and taken up in ethyl acetate. The solids were removed by filtration and the filtrate was washed twice with 1 N hydrochloric acid and brine a...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
c1ccc2c(c1)CCN2
c1ccc2c(c1)CCN2.c1ccccc1
Other
[Fe].C(C)(=O)O
null
null
O=C(O)Cc1ccc(-c2ccccc2)cc1[N+](=O)[O-]>[Fe].C(C)(=O)O>O=C1Cc2ccc(-c3ccccc3)cc2N1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-95c0514ee8dd40ee8d7b1d05041a7485
COC(=O)CC(=O)OC.COc1ccccc1-c1ccc(F)c([N+](=O)[O-])c1>>COC(=O)C(C(=O)OC)c1ccc(-c2ccccc2OC)cc1[N+](=O)[O-]
FC1=C(C=C(C=C1)C1=C(C=CC=C1)OC)[N+](=O)[O-].C(CC(=O)OC)(=O)OC.[H-].[Na+]>>COC1=C(C=CC=C1)C1=CC(=C(C=C1)C(C(=O)OC)C(=O)OC)[N+](=O)[O-]
[CH3:1][O:2][C:3](=[O:4])[CH2:5][C:6](=[O:7])[O:8][CH3:9].F[c:10]1[cH:11][cH:12][c:13](-[c:14]2[cH:15][cH:16][cH:17][cH:18][c:19]2[O:20][CH3:21])[cH:22][c:23]1[N+:24](=[O:25])[O-:26]>>[CH3:1][O:2][C:3](=[O:4])[CH:5]([C:6](=[O:7])[O:8][CH3:9])[c:10]1[cH:11][cH:12][c:13](-[c:14]2[cH:15][cH:16][cH:17][cH:18][c:19]2[O:20][...
COC(=O)CC(=O)OC.COc1ccccc1-c1ccc(F)c([N+](=O)[O-])c1
COC(=O)C(C(=O)OC)c1ccc(-c2ccccc2OC)cc1[N+](=O)[O-]
null
null
CS(=O)C
C-C Coupling
OtherReaction
5a1171068c2a10d196160f01101b1c97354196d6923cfc455c6b686284d6c6f2
c0fb657475d92a5e1ab643a3f03921ebe4d047c8d805f98b012a5df3f9fb1f6c
c1ccc(-c2ccccc2)cc1
F-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[#7;+:5]):[c:6].[C;D1;H3:7]-[#8:8]-[C:9](=[O;D1;H0:10])-[CH2;D2;+0:11]-[C:12](=[O;D1;H0:13])-[#8:14]-[C;D1;H3:15]>>[#7;+:5]-[c:4](:[c:6]):[c;H0;D3;+0:1](-[CH;D3;+0:11](-[C:9](=[O;D1;H0:10])-[#8:8]-[C;D1;H3:7])-[C:12](=[O;D1;H0:13])-[#8:14]-[C;D1;H3:15]):[c:2]:[c:3]
null
[]
100
CELSIUS
null
null
Dimethyl malonate (14 mL) was added dropwise to 2.9 g of sodium hydride suspended in 50 mL of dimethylsulfoxide. The mixture was heated at 100° C. for 15 minutes and cooled to room temperature. Crude 4-fluoro-2′-methoxy-3-nitrobiphenyl in 60 mL of dimethylsulfoxide was added and the mixture was heated at 100° C. for 2 ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Ester
Ester.Ester
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1
HF
CS(=O)C
100
null
COC(=O)CC(=O)OC.COc1ccccc1-c1ccc(F)c([N+](=O)[O-])c1>CS(=O)C>COC(=O)C(C(=O)OC)c1ccc(-c2ccccc2OC)cc1[N+](=O)[O-]
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-47b2bfe7d4eb4a989b1b246f46f8e9fa
COc1ccccc1-c1ccc(CC(=O)O)c([N+](=O)[O-])c1>>COc1ccccc1-c1ccc2c(c1)NC(=O)C2
COC1=C(C=CC=C1)C1=CC(=C(C=C1)CC(=O)O)[N+](=O)[O-]>>COC1=C(C=CC=C1)C1=CC=C2CC(NC2=C1)=O
O=[N+:15]([O-])[c:13]1[c:12]([CH2:18][C:16](O)=[O:17])[cH:11][cH:10][c:9](-[c:8]2[c:3]([O:2][CH3:1])[cH:4][cH:5][cH:6][cH:7]2)[cH:14]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][cH:7][c:8]1-[c:9]1[cH:10][cH:11][c:12]2[c:13]([cH:14]1)[NH:15][C:16](=[O:17])[CH2:18]2
COc1ccccc1-c1ccc(CC(=O)O)c([N+](=O)[O-])c1
COc1ccccc1-c1ccc2c(c1)NC(=O)C2
null
[Fe]
C(C)(=O)O
Functional Group Interconversion
OtherReaction
e98c7e13a0e22318df8d26b28a8117bfb6ce0313bb5b14de92a87461040b8923
98c112fcc8dd821704dc378798368c2081a2acc574356674c70af3e59954ee0d
O=C1Cc2ccc(-c3ccccc3)cc2N1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[c:4]:[c:5](-[N+;H0;D3:6](=O)-[O-]):[c:7]>>[O;D1;H0:2]=[C;H0;D3;+0:1]1-[C:3]-[c:4]:[c:5](:[c:7])-[NH;D2;+0:6]-1
69
[{"value": 69.0, "product": "COC1=C(C=CC=C1)C1=CC=C2CC(NC2=C1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 66.2, "product": "COC1=C(C=CC=C1)C1=CC=C2CC(NC2=C1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
null
null
Iron chips (5 g) were added in one portion to 9.8 g of 2′-methoxy-3-nitrobiphenyl-4-acetic acid in 50 mL of glacial acetic acid and heated to 100° C. for 3 hours. The reaction mixture was concentrated to dryness, sonicated in ethyl acetate and filtered to remove the insolubles. The filtrate was washed twice with 1 N hy...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
c1ccc2c(c1)CCN2
c1ccccc1.c1ccc2c(c1)CCN2
Other
[Fe].C(C)(=O)O
100
null
COc1ccccc1-c1ccc(CC(=O)O)c([N+](=O)[O-])c1>[Fe].C(C)(=O)O>COc1ccccc1-c1ccc2c(c1)NC(=O)C2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0aedcfaa8c0a46d5b70cbff208230660
COc1cccc(B(O)O)c1.O=[N+]([O-])c1cc(Br)ccc1F>>COc1cccc(-c2ccc(F)c([N+](=O)[O-])c2)c1
COC=1C=C(C=CC1)B(O)O.BrC=1C=CC(=C(C1)[N+](=O)[O-])F.C([O-])([O-])=O.[Na+].[Na+]>>FC1=C(C=C(C=C1)C1=CC(=CC=C1)OC)[N+](=O)[O-]
OB(O)[c:7]1[cH:6][cH:5][cH:4][c:3]([O:2][CH3:1])[cH:18]1.Br[c:8]1[cH:9][cH:10][c:11]([F:12])[c:13]([N+:14](=[O:15])[O-:16])[cH:17]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][c:11]([F:12])[c:13]([N+:14](=[O:15])[O-:16])[cH:17]2)[cH:18]1
COc1cccc(B(O)O)c1.O=[N+]([O-])c1cc(Br)ccc1F
COc1cccc(-c2ccc(F)c([N+](=O)[O-])c2)c1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.C1(=CC=CC=C1)C
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccccc2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:5]:[c:4]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:2]:[c:3]
77
[{"value": 77.0, "product": "FC1=C(C=C(C=C1)C1=CC(=CC=C1)OC)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 76.5, "product": "FC1=C(C=C(C=C1)C1=CC(=CC=C1)OC)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Tetrakis(triphenylphosphine)palladium (0.7 g) was added to a mixture of 3.8 g of 3-methoxyphenylboronic acid, 5 g of 5-bromo-2-fluoronitrobenzene and 11 mL of 2 M sodium carbonate solution in 100 mL of toluene. The mixture was heated to reflux for 2 hours, diluted with water and extracted with ethyl acetate. The ethyl ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.C1(=CC=CC=C1)C
null
null
COc1cccc(B(O)O)c1.O=[N+]([O-])c1cc(Br)ccc1F>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.C1(=CC=CC=C1)C>COc1cccc(-c2ccc(F)c([N+](=O)[O-])c2)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ec1c217554b04edcb37dde22329173fb
COc1cccc(-c2ccc(CC(=O)O)c([N+](=O)[O-])c2)c1>>COc1cccc(-c2ccc3c(c2)NC(=O)C3)c1
COC=1C=C(C=CC1)C1=CC(=C(C=C1)CC(=O)O)[N+](=O)[O-]>>COC=1C=C(C=CC1)C1=CC=C2CC(NC2=C1)=O
O=[N+:14]([O-])[c:12]1[c:11]([CH2:17][C:15](O)=[O:16])[cH:10][cH:9][c:8](-[c:7]2[cH:6][cH:5][cH:4][c:3]([O:2][CH3:1])[cH:18]2)[cH:13]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][c:11]3[c:12]([cH:13]2)[NH:14][C:15](=[O:16])[CH2:17]3)[cH:18]1
COc1cccc(-c2ccc(CC(=O)O)c([N+](=O)[O-])c2)c1
COc1cccc(-c2ccc3c(c2)NC(=O)C3)c1
null
[Pd]
CO
Functional Group Interconversion
OtherReaction
e98c7e13a0e22318df8d26b28a8117bfb6ce0313bb5b14de92a87461040b8923
98c112fcc8dd821704dc378798368c2081a2acc574356674c70af3e59954ee0d
O=C1Cc2ccc(-c3ccccc3)cc2N1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[c:4]:[c:5](-[N+;H0;D3:6](=O)-[O-]):[c:7]>>[O;D1;H0:2]=[C;H0;D3;+0:1]1-[C:3]-[c:4]:[c:5](:[c:7])-[NH;D2;+0:6]-1
75
[{"value": 75.0, "product": "COC=1C=C(C=CC1)C1=CC=C2CC(NC2=C1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 69.3, "product": "COC=1C=C(C=CC1)C1=CC=C2CC(NC2=C1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
3′-Methoxy-3-nitrobiphenyl-4-acetic acid (5.2 g) was dissolved in methanol and hydrogenated over 0.8 g of 10% palladium on carbon for 3 hours at room temperature. The catalyst was removed by filtration, washed with methanol and the filtrates combined and concentrated to give a brown solid. The solid was purified by col...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
c1ccc2c(c1)CCN2
c1ccccc1.c1ccc2c(c1)CCN2
Other
[Pd].CO
null
null
COc1cccc(-c2ccc(CC(=O)O)c([N+](=O)[O-])c2)c1>[Pd].CO>COc1cccc(-c2ccc3c(c2)NC(=O)C3)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-40cd27683e8240bf9bb68ae563315f45
COc1ccc(B(O)O)cc1.O=[N+]([O-])c1cc(Br)ccc1F>>COc1ccc(-c2ccc(F)c([N+](=O)[O-])c2)cc1
COC1=CC=C(C=C1)B(O)O.BrC=1C=CC(=C(C1)[N+](=O)[O-])F.C([O-])([O-])=O.[Na+].[Na+]>>FC1=C(C=C(C=C1)C1=CC=C(C=C1)OC)[N+](=O)[O-]
OB(O)[c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:18][cH:17]1.Br[c:7]1[cH:8][cH:9][c:10]([F:11])[c:12]([N+:13](=[O:14])[O-:15])[cH:16]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([F:11])[c:12]([N+:13](=[O:14])[O-:15])[cH:16]2)[cH:17][cH:18]1
COc1ccc(B(O)O)cc1.O=[N+]([O-])c1cc(Br)ccc1F
COc1ccc(-c2ccc(F)c([N+](=O)[O-])c2)cc1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
C1(=CC=CC=C1)C.C(C)O
C-C Coupling
Suzuki coupling with boronic acids
d79a78c79f0c392f0911481acf5c300cc98205269acdb93c24fb610a61c4c868
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccccc2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:4]:[c:5]
null
[]
null
null
null
null
Tetrakis(triphenylphosphine)palladium (1 g) was added to a mixture of 5 g of 4-methoxyphenylboronic acid, 6.6 g of 5-bromo-2-fluoronitrobenzene and 30 mL of 2 M sodium carbonate solution in 50 mL of toluene and 50 mL of ethanol. The mixture was heated to reflux for 2 hours, concentrated, and the residue extracted twice...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
c1ccccc1.c1ccccc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C1(=CC=CC=C1)C.C(C)O
null
null
COc1ccc(B(O)O)cc1.O=[N+]([O-])c1cc(Br)ccc1F>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C1(=CC=CC=C1)C.C(C)O>COc1ccc(-c2ccc(F)c([N+](=O)[O-])c2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c9b374d7d7684b1a8263159d26e065d4
COc1ccc(-c2ccc(C(C(=O)[O-])C(=O)[O-])c([N+](=O)[O-])c2)cc1>>COc1ccc(-c2ccc(CC(=O)O)c([N+](=O)[O-])c2)cc1
COC1=CC=C(C=C1)C1=CC(=C(C=C1)C(C(=O)[O-])C(=O)[O-])[N+](=O)[O-]>>COC1=CC=C(C=C1)C1=CC(=C(C=C1)CC(=O)O)[N+](=O)[O-]
O=C([O-])[CH:11]([c:10]1[cH:9][cH:8][c:7](-[c:6]2[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:21][cH:20]2)[cH:19][c:15]1[N+:16](=[O:17])[O-:18])[C:12](=[O:13])[O-:14]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]([CH2:11][C:12](=[O:13])[OH:14])[c:15]([N+:16](=[O:17])[O-:18])[cH:19]2)[cH:20][cH:21]1
COc1ccc(-c2ccc(C(C(=O)[O-])C(=O)[O-])c([N+](=O)[O-])c2)cc1
COc1ccc(-c2ccc(CC(=O)O)c([N+](=O)[O-])c2)cc1
null
null
Cl
Reduction
OtherReaction
65edb34f59b888c9ecb87d6c8e9fd76d082de6afc49403d96c457f834c73148e
222e2311064b3cb906d6bdeba44711f5dada050c096bbbcc7b35038975f228e8
c1ccc(-c2ccccc2)cc1
O=C(-[O-])-[CH;D3;+0:1](-[C:2](-[O-;H0;D1:3])=[O;D1;H0:4])-[c:5](:[c:6]):[c:7]>>[O;D1;H0:4]=[C:2](-[OH;D1;+0:3])-[CH2;D2;+0:1]-[c:5](:[c:6]):[c:7]
null
[]
null
null
null
null
Crude 4′-methoxy-3-nitro-biphenyl-4-malonate was heated at 100° C. in 60 mL of 6 N hydrochloric acid for 15 hours and cooled. The precipitate was collected by filtration, washed with water and hexane, and dried to give 7.2 g of crude 4′-methoxy-3-nitrobiphenyl-4-acetic acid as a light tan solid. Conditions: See reactio...
10.6084/m9.figshare.5104873.v1
null
null
Carboxylic acid
null
null
c1ccccc1.c1ccccc1
Other
Cl
null
null
COc1ccc(-c2ccc(C(C(=O)[O-])C(=O)[O-])c([N+](=O)[O-])c2)cc1>Cl>COc1ccc(-c2ccc(CC(=O)O)c([N+](=O)[O-])c2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c22e35016f334ef985010b8adb49a67a
COc1ccc(-c2ccc(CC(=O)O)c([N+](=O)[O-])c2)cc1>>COc1ccc(-c2ccc3c(c2)NC(=O)C3)cc1
COC1=CC=C(C=C1)C1=CC(=C(C=C1)CC(=O)O)[N+](=O)[O-]>>COC1=CC=C(C=C1)C1=CC=C2CC(NC2=C1)=O
O=[N+:13]([O-])[c:11]1[c:10]([CH2:16][C:14](O)=[O:15])[cH:9][cH:8][c:7](-[c:6]2[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:18][cH:17]2)[cH:12]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]3[c:11]([cH:12]2)[NH:13][C:14](=[O:15])[CH2:16]3)[cH:17][cH:18]1
COc1ccc(-c2ccc(CC(=O)O)c([N+](=O)[O-])c2)cc1
COc1ccc(-c2ccc3c(c2)NC(=O)C3)cc1
null
[Fe]
C(C)(=O)O
Functional Group Interconversion
OtherReaction
e98c7e13a0e22318df8d26b28a8117bfb6ce0313bb5b14de92a87461040b8923
98c112fcc8dd821704dc378798368c2081a2acc574356674c70af3e59954ee0d
O=C1Cc2ccc(-c3ccccc3)cc2N1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[c:4]:[c:5](-[N+;H0;D3:6](=O)-[O-]):[c:7]>>[O;D1;H0:2]=[C;H0;D3;+0:1]1-[C:3]-[c:4]:[c:5](:[c:7])-[NH;D2;+0:6]-1
54
[{"value": 54.0, "product": "COC1=CC=C(C=C1)C1=CC=C2CC(NC2=C1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 45.0, "product": "COC1=CC=C(C=C1)C1=CC=C2CC(NC2=C1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
null
null
Iron chips (3.6 g) were added in one portion to 7.2 g of 4′-methoxy-3-nitrobiphenyl-4-acetic acid in 50 mL of glacial acetic acid and heated at 100° C. overnight. The reaction mixture was concentrated to dryness, sonicated in ethyl acetate and filtered to remove the insolubles. The filtrate was washed twice with 1 N hy...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Nitro group
Secondary amide
null
c1ccc2c(c1)CCN2
c1ccccc1.c1ccc2c(c1)CCN2
Other
[Fe].C(C)(=O)O
100
null
COc1ccc(-c2ccc(CC(=O)O)c([N+](=O)[O-])c2)cc1>[Fe].C(C)(=O)O>COc1ccc(-c2ccc3c(c2)NC(=O)C3)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-be65052310f24bffa8ad90b56f56a7dc
COc1ccc(N)cc1Cl.O=C1Cc2c(cccc2C(=O)O)N1>>COc1ccc(NC(=O)c2cccc3c2CC(=O)N3)cc1Cl
O=C1NC=2C=CC=C(C2C1)C(=O)O.ClC=1C=C(C=CC1OC)N.F[P-](F)(F)(F)(F)F.N1(N=NC2=C1C=CC=C2)O[P+](N(C)C)(N(C)C)N(C)C>>ClC=1C=C(C=CC1OC)NC(=O)C=1C=2CC(NC2C=CC1)=O
[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([NH2:7])[cH:20][c:21]1[Cl:22].O[C:8](=[O:9])[c:10]1[cH:11][cH:12][cH:13][c:14]2[c:15]1[CH2:16][C:17](=[O:18])[NH:19]2>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([NH:7][C:8](=[O:9])[c:10]2[cH:11][cH:12][cH:13][c:14]3[c:15]2[CH2:16][C:17](=[O:18])[NH:19]3)[cH:20][c:21]1[Cl:22]
COc1ccc(N)cc1Cl.O=C1Cc2c(cccc2C(=O)O)N1
COc1ccc(NC(=O)c2cccc3c2CC(=O)N3)cc1Cl
null
CN(C1=CC=NC=C1)C
CN(C=O)C.C(C)(=O)OCC
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C1Cc2c(cccc2C(=O)Nc2ccccc2)N1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9])-[c:3](:[c:4]):[c:5]
null
[]
null
null
72
HOUR
To a solution of 2-oxo-2,3-dihydro-1H-indole-4-carboxylic acid (200 mg, 1.13 mmol) and 3-chloro-4-methoxy-phenylamine (178 mg, 1.13 mmol) in dimethylformamide (15 mL) at room temperature benzotriazol-1-yloxytris(dimethylamino)phosphonium hexafluorophosphate (BOP reagent 997 mg, 2.26 mmol) was added followed by 4-dimeth...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccc2c(c1)CCN2
HO-
CN(C1=CC=NC=C1)C.CN(C=O)C.C(C)(=O)OCC
null
72
COc1ccc(N)cc1Cl.O=C1Cc2c(cccc2C(=O)O)N1>CN(C1=CC=NC=C1)C.CN(C=O)C.C(C)(=O)OCC>COc1ccc(NC(=O)c2cccc3c2CC(=O)N3)cc1Cl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-086f2bea67084563aeccecbb77a52574
CCN.O=C1Cc2c(cccc2C(=O)O)N1>>CCNC(=O)c1cccc2c1CC(=O)N2
C(C)N.C(=O)(O)C1=C2CC(NC2=CC=C1)=O.C1CCN(C1)[P+](N2CCCC2)(N3CCCC3)ON4C5=C(C=CC=C5)N=N4.F[P-](F)(F)(F)(F)F>>C(C)NC(=O)C=1C=2CC(NC2C=CC1)=O
[CH3:1][CH2:2][NH2:3].O[C:4](=[O:5])[c:6]1[cH:7][cH:8][cH:9][c:10]2[c:11]1[CH2:12][C:13](=[O:14])[NH:15]2>>[CH3:1][CH2:2][NH:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][cH:9][c:10]2[c:11]1[CH2:12][C:13](=[O:14])[NH:15]2
CCN.O=C1Cc2c(cccc2C(=O)O)N1
CCNC(=O)c1cccc2c1CC(=O)N2
null
CN(C1=CC=NC=C1)C
CN(C=O)C
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C1Cc2ccccc2N1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C;D1;H3:6]-[C:7]-[NH2;D1;+0:8]>>[C;D1;H3:6]-[C:7]-[NH;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
65.3
[{"value": 65.0, "product": "C(C)NC(=O)C=1C=2CC(NC2C=CC1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 65.3, "product": "C(C)NC(=O)C=1C=2CC(NC2C=CC1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
6
HOUR
Ethylamine (2.1 mL of 2.0 M solution in tetrahydrofuran, 4.2 mmol) was added dropwise to a suspension of 4-carboxy-2-oxindole (380 mg, 2.1 mmol) in dimethylformamide (8 mL), followed by 4-dimethylaminopyridine (385 mg, 3.15 mmol) and PyBOP (2.185 g, 4.2 mmol). The mixture was stirred at room temperature for 6 hrs. The ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccc2c(c1)CCN2
HO-
CN(C1=CC=NC=C1)C.CN(C=O)C
null
6
CCN.O=C1Cc2c(cccc2C(=O)O)N1>CN(C1=CC=NC=C1)C.CN(C=O)C>CCNC(=O)c1cccc2c1CC(=O)N2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b5d42876c3b7492fa6b2aad18e23ba11
O=Cc1ccccc1.OCCO>>c1ccc(C2OCCO2)cc1
C(C1=CC=CC=C1)=O.C(CO)O.O>>C1(=CC=CC=C1)C1OCCO1
[cH:1]1[cH:2][cH:3][c:4]([CH:5]=[O:6])[cH:10][cH:11]1.O[CH2:7][CH2:8][OH:9]>>[cH:1]1[cH:2][cH:3][c:4]([CH:5]2[O:6][CH2:7][CH2:8][O:9]2)[cH:10][cH:11]1
O=Cc1ccccc1.OCCO
c1ccc(C2OCCO2)cc1
null
O.C1(=CC=C(C=C1)S(=O)(=O)O)C
C1=CC=CC=C1
Heteroatom Alkylation and Arylation
OtherReaction
fe0fbb45a87f24c1e456c6b4e41101562cd8f0af3ec376bb6115e7c1555d997b
7ac65b5a5f576337ce8e86e0130eb9b4757ca21b2419a0e82bbdfd5def30ee73
c1ccc(C2OCCO2)cc1
O-[CH2;D2;+0:1]-[C:2]-[OH;D1;+0:3].[O;H0;D1;+0:4]=[CH;D2;+0:5]-[c:6](:[c:7]):[c:8]>>[c:7]:[c:6](-[CH;D3;+0:5]1-[O;H0;D2;+0:4]-[CH2;D2;+0:1]-[C:2]-[O;H0;D2;+0:3]-1):[c:8]
89
[{"value": 89.0, "product": "C1(=CC=CC=C1)C1OCCO1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 89.0, "product": "C1(=CC=CC=C1)C1OCCO1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A 500-mL three-necked flask equipped with a reflux condenser having a Dean-Stark water trap was charged with 5.0 g of benzaldehyde, 29.3 g of ethylene glycol, 0.09 g of p-toluenesulfonic acid monohydrate and 250 mL of benzene, and the contents were refluxed for 21 h. The resultant reaction solution was allowed to stand...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary alcohol.Primary alcohol
Ether.Ether
null
C1COCO1
c1ccccc1.C1COCO1
HO-
O.C1(=CC=C(C=C1)S(=O)(=O)O)C.C1=CC=CC=C1
null
null
O=Cc1ccccc1.OCCO>O.C1(=CC=C(C=C1)S(=O)(=O)O)C.C1=CC=CC=C1>c1ccc(C2OCCO2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-93912b0f9c4e4dadbfc0baf5ed7206e6
O=Cc1ccccc1.OCCO>>c1ccc(C2OCCO2)cc1
C(C1=CC=CC=C1)=O.C(CO)O.O>>C1(=CC=CC=C1)C1OCCO1
[cH:1]1[cH:2][cH:3][c:4]([CH:5]=[O:6])[cH:10][cH:11]1.O[CH2:7][CH2:8][OH:9]>>[cH:1]1[cH:2][cH:3][c:4]([CH:5]2[O:6][CH2:7][CH2:8][O:9]2)[cH:10][cH:11]1
O=Cc1ccccc1.OCCO
c1ccc(C2OCCO2)cc1
null
O.C1(=CC=C(C=C1)S(=O)(=O)O)C
C1=CC=CC=C1
Heteroatom Alkylation and Arylation
OtherReaction
fe0fbb45a87f24c1e456c6b4e41101562cd8f0af3ec376bb6115e7c1555d997b
7ac65b5a5f576337ce8e86e0130eb9b4757ca21b2419a0e82bbdfd5def30ee73
c1ccc(C2OCCO2)cc1
O-[CH2;D2;+0:1]-[C:2]-[OH;D1;+0:3].[O;H0;D1;+0:4]=[CH;D2;+0:5]-[c:6](:[c:7]):[c:8]>>[c:7]:[c:6](-[CH;D3;+0:5]1-[O;H0;D2;+0:4]-[CH2;D2;+0:1]-[C:2]-[O;H0;D2;+0:3]-1):[c:8]
89
[{"value": 89.0, "product": "C1(=CC=CC=C1)C1OCCO1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 89.0, "product": "C1(=CC=CC=C1)C1OCCO1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A 500-mL three-necked flask equipped with a reflux condenser having a Dean-Stark water trap was charged with 5.0 g of benzaldehyde, 29.3 g of ethylene glycol, 0.09 g of p-toluenesulfonic acid monohydrate and 250 mL of benzene, and the contents were refluxed for 21 h. The resultant reaction solution was allowed to stand...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary alcohol.Primary alcohol
Ether.Ether
null
C1COCO1
c1ccccc1.C1COCO1
HO-
O.C1(=CC=C(C=C1)S(=O)(=O)O)C.C1=CC=CC=C1
null
null
O=Cc1ccccc1.OCCO>O.C1(=CC=C(C=C1)S(=O)(=O)O)C.C1=CC=CC=C1>c1ccc(C2OCCO2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-fecd8c4325a044fe9432bcdb6bfcaf63
C=CC.Oc1c(-c2ccc3c(c2)CCCC3)ccc2c1CCCC2>>CC(C)c1cc2c(c(O)c1-c1ccc3c(c1)CCCC3)CCCC2
C=1(C(=CC=C2CCCCC12)C1=CC=2CCCCC2C=C1)O.C=CC.C=1(C(=CC=C2CCCCC12)C1=CC=2CCCCC2C=C1)O>>C(C)(C)C1=C(C(=C2CCCCC2=C1)O)C1=CC=2CCCCC2C=C1
[CH2:1]=[CH:2][CH3:3].[cH:4]1[cH:5][c:6]2[c:7]([c:8]([OH:9])[c:10]1-[c:11]1[cH:12][cH:13][c:14]3[c:15]([cH:16]1)[CH2:17][CH2:18][CH2:19][CH2:20]3)[CH2:21][CH2:22][CH2:23][CH2:24]2>>[CH3:1][CH:2]([CH3:3])[c:4]1[cH:5][c:6]2[c:7]([c:8]([OH:9])[c:10]1-[c:11]1[cH:12][cH:13][c:14]3[c:15]([cH:16]1)[CH2:17][CH2:18][CH2:19][CH2...
C=CC.Oc1c(-c2ccc3c(c2)CCCC3)ccc2c1CCCC2
CC(C)c1cc2c(c(O)c1-c1ccc3c(c1)CCCC3)CCCC2
null
O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.P.[W].[W].[W].[W].[W].[W].[W].[W].[W].[W].[W].[W]
C=1(C(=CC=CC1)C)C
C-C Coupling
Friedel-Crafts alkylation
ec8f21b326d83472ee4b10e7d20a55a7273fffbc535eac62ffaaea718d36de52
48297e5b607b4624d5b08506879ba8f9dd47fb272c10888542fa01ef83829ef2
c1cc2c(cc1-c1ccc3c(c1)CCCC3)CCCC2
[C;D1;H3:1]-[CH;D2;+0:2]=[CH2;D1;+0:3].[c:4]-[c:5](:[c:6]):[cH;D2;+0:7]:[c:8]:[c:9]>>[C;D1;H3:1]-[CH;D3;+0:2](-[CH3;D1;+0:3])-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:5](-[c:4]):[c:6]
42
[{"value": 42.0, "product": "C(C)(C)C1=C(C(=C2CCCCC2=C1)O)C1=CC=2CCCCC2C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
140
CELSIUS
null
null
A mixture of 5,5′,6,6′,7,7′,8,8′-octahydro-2,2′-binaphthol (30.0 g), xylene (5 ml) and phosphotungstic acid (1.5 g) was heated to 140° C. To the mixture was added propylene (8.9 g) slowly via a dry-ice condenser. GC analysis of the reaction mixture indicated that 98% conversion of the 5,5′,6,6′,7,7′,8,8′-octahydro-2,2′...
10.6084/m9.figshare.5104873.v1
null
Vinyl
null
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2.c1ccc2c(c1)CCCC2
null
O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.P.[W].[W].[W].[W].[W].[W].[W].[W].[W].[W].[W].[W].C=1(C(=CC=CC1)C)C
140
null
C=CC.Oc1c(-c2ccc3c(c2)CCCC3)ccc2c1CCCC2>O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.P.[W].[W].[W].[W].[W].[W].[W].[W].[W].[W].[W].[W].C=1(C(=CC=CC1)C)C>CC(C)c1cc2c(c(O)c1-c1ccc3c(c1)CCCC3)CCCC2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-366fafc4eb344e6ebc2c03201dcde3fe
C=CC.Clc1ccc(Cl)cc1.Oc1c(-c2ccc3c(c2)CCCC3)ccc2c1CCCC2>>CC(C)c1cc2c(cc1-c1c(C(C)C)cc3c(c1O)CCCC3)CCCC2
C=1(C(=CC=C2CCCCC12)C1=CC=2CCCCC2C=C1)O.C1=CC(=CC=C1Cl)Cl.C=CC>>C(C)(C)C1=C(C(=C2CCCCC2=C1)O)C1=CC=2CCCCC2C=C1C(C)C
[CH:2](=[CH2:3])[CH3:14].Clc1c[cH:13][c:12](Cl)c[cH:1]1.[cH:4]1[cH:5][c:6]2[c:7]([cH:8][c:9]1-[c:10]1[cH:11][cH:15][c:16]3[c:17]([c:18]1[OH:19])[CH2:20][CH2:21][CH2:22][CH2:23]3)[CH2:24][CH2:25][CH2:26][CH2:27]2>>[CH3:1][CH:2]([CH3:3])[c:4]1[cH:5][c:6]2[c:7]([cH:8][c:9]1-[c:10]1[c:11]([CH:12]([CH3:13])[CH3:14])[cH:15][...
C=CC.Clc1ccc(Cl)cc1.Oc1c(-c2ccc3c(c2)CCCC3)ccc2c1CCCC2
CC(C)c1cc2c(cc1-c1c(C(C)C)cc3c(c1O)CCCC3)CCCC2
null
O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.P.[W].[W].[W].[W].[W].[W].[W].[W].[W].[W].[W].[W]
null
C-C Coupling
OtherReaction
22b6bb8d84b60d31f45107e068d2c7f6a47a8bbb4ec121f47047d6d567bb8a05
6085f512e278c1c48c257e40fa8895f511b6c14f22cbc4a119e27edc859a5be0
c1cc2c(cc1-c1ccc3c(c1)CCCC3)CCCC2
Cl-[c;H0;D3;+0:1]1:[cH;D2;+0:2]:c:c(-Cl):[cH;D2;+0:3]:c:1.[CH2;D1;+0:4]=[CH;D2;+0:5]-[CH3;D1;+0:6].[c:7]:[c:8]:[cH;D2;+0:9]:[c:10](-[c:11](:[c:12]):[cH;D2;+0:13]:[c:14]:[c:15]):[c:16]>>[CH3;D1;+0:2]-[CH;D3;+0:1](-[CH3;D1;+0:6])-[c;H0;D3;+0:9](:[c:8]:[c:7]):[c:10](-[c:11](:[c:12]):[c;H0;D3;+0:13](-[CH;D3;+0:5](-[CH3;D1;...
null
[]
130
CELSIUS
null
null
A mixture of 5,5′,6,6′,7,7′,8,8′-octahydro-2,2′-binaphthol (44.0 g), dichlorobenzene (10 ml) and phosphotungstic acid (2.3 g) was heated to 130° C. To the mixture was added excess propylene via a dry-ice condenser. The reaction was monitored by GC analysis. The reaction mixture contained 6% of monoisopropylated product...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide.Vinyl
null
c1ccccc1.c1ccc2c(c1)CCCC2.c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2.c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2.c1ccc2c(c1)CCCC2
Other
O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.P.[W].[W].[W].[W].[W].[W].[W].[W].[W].[W].[W].[W]
130
null
C=CC.Clc1ccc(Cl)cc1.Oc1c(-c2ccc3c(c2)CCCC3)ccc2c1CCCC2>O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.P.[W].[W].[W].[W].[W].[W].[W].[W].[W].[W].[W].[W]>CC(C)c1cc2c(cc1-c1c(C(C)C)cc3c(c1O)CCCC3)CCCC2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-77786d6651e545b5b9146ffe454cfdf6
C1=CCCC1.Oc1c(-c2ccc3c(c2)CCCC3)ccc2c1CCCC2>>Oc1c2c(cc(C3CCCC3)c1-c1cc3c(cc1C1CCCC1)CCCC3)CCCC2
C=1(C(=CC=C2CCCCC12)C1=CC=2CCCCC2C=C1)O.C1=CCCC1>>C1(CCCC1)C1=C(C(=C2CCCCC2=C1)O)C1=CC=2CCCCC2C=C1C1CCCC1
[CH:19]1=[CH:20][CH2:21][CH2:22][CH2:23]1.[OH:1][c:2]1[c:3]2[c:4]([cH:5][cH:6][c:12]1-[c:7]1[cH:14][c:13]3[c:15]([cH:26][cH:25]1)[CH2:11][CH2:10][CH2:9][CH2:8]3)[CH2:28][CH2:29][CH2:30][CH2:31]2>>[OH:1][c:2]1[c:3]2[c:4]([cH:5][c:6]([CH:7]3[CH2:8][CH2:9][CH2:10][CH2:11]3)[c:12]1-[c:13]1[cH:14][c:15]3[c:16]([cH:17][c:18]...
C1=CCCC1.Oc1c(-c2ccc3c(c2)CCCC3)ccc2c1CCCC2
Oc1c2c(cc(C3CCCC3)c1-c1cc3c(cc1C1CCCC1)CCCC3)CCCC2
null
O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.P.[W].[W].[W].[W].[W].[W].[W].[W].[W].[W].[W].[W]
null
C-C Coupling
OtherReaction
53496ddc706f3c3b0b9bdeb7dff6105fa36d9e1fa2ad53fb753e3e4cb9578828
410ec9b1cc243569e4ff568c248f0b402403802e002b4018f576af3f6960507b
c1c2c(cc(C3CCCC3)c1-c1cc3c(cc1C1CCCC1)CCCC3)CCCC2
[C:1]1-[C:2]-[C:3]-[CH;D2;+0:4]=[CH;D2;+0:5]-1.[O;D1;H1:6]-[c:7]1:[c:8]:[c:9]:[c:10]:[cH;D2;+0:11]:[c;H0;D3;+0:12]:1-[c;H0;D3;+0:13]1:[cH;D2;+0:14]:[c;H0;D3;+0:15]2:[c;H0;D3;+0:16](:[cH;D2;+0:17]:[cH;D2;+0:18]:1)-[CH2;D2;+0:19]-[C:20]-[C:21]-[CH2;D2;+0:22]-2>>[O;D1;H1:6]-[c:7]1:[c:8]:[c:9]:[c:10]:[c;H0;D3;+0:11](-[CH;D...
42
[{"value": 42.0, "product": "C1(CCCC1)C1=C(C(=C2CCCCC2=C1)O)C1=CC=2CCCCC2C=C1C1CCCC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 41.3, "product": "C1(CCCC1)C1=C(C(=C2CCCCC2=C1)O)C1=CC=2CCCCC2C=C1C1CCCC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 5,5′,6,6′,7,7′,8,8′-octahydro-2,2′-binapthol (48 g), phosphotungstic acid (2.4 g) and cyclopentene (58 g) was charged into a Hastelloy reactor. The reactor was heated to 180 C for 40 hours. The mixture was purified by column chromatography (silica gel, eluting with 2% ethyl acetate/hexane) to yield 29.5 g ...
10.6084/m9.figshare.5104873.v1
null
null
null
C1=CCCC1.c1ccc2c(c1)CCCC2.c1ccc2c(c1)CCCC2
C1CCCC1.C1CCCC1.c1ccc2c(c1)CCCC2.c1ccc2c(c1)CCCC2
C1CCCC1.C1CCCC1.c1ccc2c(c1)CCCC2.c1ccc2c(c1)CCCC2
Other
O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.P.[W].[W].[W].[W].[W].[W].[W].[W].[W].[W].[W].[W]
null
null
C1=CCCC1.Oc1c(-c2ccc3c(c2)CCCC3)ccc2c1CCCC2>O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.O.P.[W].[W].[W].[W].[W].[W].[W].[W].[W].[W].[W].[W]>Oc1c2c(cc(C3CCCC3)c1-c1cc3c(cc1C1CCCC1)CCCC3)CCCC2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-04a94cb311e24ec1addae5f01600a743
CC(C)OS(C)(=O)=O.Oc1c(-c2ccc3c(c2)CCCC3)ccc2c1CCCC2>>CC(C)c1cc2c(c(O)c1-c1ccc3c(c1)CCCC3)CCCC2
C=1(C(=CC=C2CCCCC12)C1=CC=2CCCCC2C=C1)O.CS(=O)(=O)OC(C)C>>C(C)(C)C1=C(C(=C2CCCCC2=C1)O)C1=CC=2CCCCC2C=C1
CS(=O)(=O)O[CH:2]([CH3:1])[CH3:3].[cH:4]1[cH:5][c:6]2[c:7]([c:8]([OH:9])[c:10]1-[c:11]1[cH:12][cH:13][c:14]3[c:15]([cH:16]1)[CH2:17][CH2:18][CH2:19][CH2:20]3)[CH2:21][CH2:22][CH2:23][CH2:24]2>>[CH3:1][CH:2]([CH3:3])[c:4]1[cH:5][c:6]2[c:7]([c:8]([OH:9])[c:10]1-[c:11]1[cH:12][cH:13][c:14]3[c:15]([cH:16]1)[CH2:17][CH2:18]...
CC(C)OS(C)(=O)=O.Oc1c(-c2ccc3c(c2)CCCC3)ccc2c1CCCC2
CC(C)c1cc2c(c(O)c1-c1ccc3c(c1)CCCC3)CCCC2
null
[O-]S(=O)(=O)C(F)(F)F.[Sc+3].[O-]S(=O)(=O)C(F)(F)F.[O-]S(=O)(=O)C(F)(F)F
C(Cl)(Cl)(Cl)Cl
C-C Coupling
OtherReaction
44609fac1e6df793c8f50b67261b725863114e1015df0f037137a23bf9c07168
b041d6622af412448d337accfca176f1c793181140e2fc4a55aecc4778a24787
c1cc2c(cc1-c1ccc3c(c1)CCCC3)CCCC2
C-S(=O)(=O)-O-[CH;D3;+0:1](-[C;D1;H3:2])-[C;D1;H3:3].[c:4]-[c:5](:[c:6]):[cH;D2;+0:7]:[c:8]:[c:9]>>[C;D1;H3:2]-[CH;D3;+0:1](-[C;D1;H3:3])-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:5](-[c:4]):[c:6]
78
[{"value": 78.0, "product": "C(C)(C)C1=C(C(=C2CCCCC2=C1)O)C1=CC=2CCCCC2C=C1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
18
HOUR
A mixture of 5,5′,6,6′,7,7′,8,8′-octahydro-2,2′-binaphthol (2 g, 6.8 mmol), isopropyl methanesulfonate (5.5 mmol), scandium triflate (0.34 g, 5 mol %), and carbon tetrachloride (10 ml) was brought to reflux under argon. After 18 hours, GC indicated 65% conversion to give 78% desired product. Additional isopropyl methan...
10.6084/m9.figshare.5104873.v1
null
Mesylate
null
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2.c1ccc2c(c1)CCCC2
MsOH.HO-
[O-]S(=O)(=O)C(F)(F)F.[Sc+3].[O-]S(=O)(=O)C(F)(F)F.[O-]S(=O)(=O)C(F)(F)F.C(Cl)(Cl)(Cl)Cl
null
18
CC(C)OS(C)(=O)=O.Oc1c(-c2ccc3c(c2)CCCC3)ccc2c1CCCC2>[O-]S(=O)(=O)C(F)(F)F.[Sc+3].[O-]S(=O)(=O)C(F)(F)F.[O-]S(=O)(=O)C(F)(F)F.C(Cl)(Cl)(Cl)Cl>CC(C)c1cc2c(c(O)c1-c1ccc3c(c1)CCCC3)CCCC2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-71922025b2c742d789cbad502858e85d
CC(C)(C)O.Oc1c(-c2ccc3c(c2)CCCC3)ccc2c1CCCC2>>CC(C)(C)c1cc2c(c(O)c1-c1ccc3c(c1)CCCC3)CCCC2
C=1(C(=CC=C2CCCCC12)C1=CC=2CCCCC2C=C1)O.C(C)(C)(C)O.FC(S(=O)(=O)O)(F)F>>C(C)(C)(C)C1=C(C(=C2CCCCC2=C1)O)C1=CC=2CCCCC2C=C1
O[C:2]([CH3:1])([CH3:3])[CH3:4].[cH:5]1[cH:6][c:7]2[c:8]([c:9]([OH:10])[c:11]1-[c:12]1[cH:13][cH:14][c:15]3[c:16]([cH:17]1)[CH2:18][CH2:19][CH2:20][CH2:21]3)[CH2:22][CH2:23][CH2:24][CH2:25]2>>[CH3:1][C:2]([CH3:3])([CH3:4])[c:5]1[cH:6][c:7]2[c:8]([c:9]([OH:10])[c:11]1-[c:12]1[cH:13][cH:14][c:15]3[c:16]([cH:17]1)[CH2:18]...
CC(C)(C)O.Oc1c(-c2ccc3c(c2)CCCC3)ccc2c1CCCC2
CC(C)(C)c1cc2c(c(O)c1-c1ccc3c(c1)CCCC3)CCCC2
null
null
ClC1=C(C=CC=C1)Cl.CCOCC.O
C-C Coupling
OtherReaction
9f30c6b466cec7957c45c711887e472599839277737f74ab7afb6bbfcc2a2cf4
80806390361076ffee90cd775b1e87663148d08d65f5b27bdd06ebc36de07186
c1cc2c(cc1-c1ccc3c(c1)CCCC3)CCCC2
O-[C;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[C;D1;H3:4].[c:5]-[c:6](:[c:7]):[cH;D2;+0:8]:[c:9]:[c:10]>>[C;D1;H3:2]-[C;H0;D4;+0:1](-[C;D1;H3:3])(-[C;D1;H3:4])-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:6](-[c:5]):[c:7]
61.6
[{"value": 61.6, "product": "C(C)(C)(C)C1=C(C(=C2CCCCC2=C1)O)C1=CC=2CCCCC2C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
120
CELSIUS
null
null
A mixture of 5,5′,6,6′,7,7′,8,8′-octahydro-2,2′-binaphthol (1.0 g, 3.4 mmol), tert-butyl alcohol (1.4 g), trifluoromethanesulfonic acid (0.04 g) was dissolved in 2 ml 1,2-dichlorobenzene. The mixture was heated at 120° C. for 2.5 hours. GC showed 97% conversion to 87% mono-butylated product, and 10% bis-butylated produ...
10.6084/m9.figshare.5104873.v1
null
Tertiary alcohol
null
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2.c1ccc2c(c1)CCCC2
HO-
ClC1=C(C=CC=C1)Cl.CCOCC.O
120
null
CC(C)(C)O.Oc1c(-c2ccc3c(c2)CCCC3)ccc2c1CCCC2>ClC1=C(C=CC=C1)Cl.CCOCC.O>CC(C)(C)c1cc2c(c(O)c1-c1ccc3c(c1)CCCC3)CCCC2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4a78a9a85ece421eb143a32bead65125
C1COCCN1.CC#CCC(C)[C@H](O)/C=C/[C@@H]1[C@H]2C/C(=C/CCCC(=O)O)C[C@H]2C[C@H]1O>>CC#CCC(C)[C@H](O)/C=C/[C@@H]1[C@H]2C/C(=C/CCCCN3CCOCC3)C[C@H]2C[C@H]1O
[Cl-].[NH4+].C(=O)(O)CCC\C=C\1/C[C@H]2C[C@H]([C@@H]([C@H]2C1)\C=C\[C@H](C(CC#CC)C)O)O.C(=O)(N1C=NC=C1)N1C=NC=C1.N1CCOCC1>>O1CCN(CC1)CCCC\C=C\1/C[C@H]2C[C@H]([C@@H]([C@H]2C1)\C=C\[C@H](C(CC#CC)C)O)O
[NH:20]1[CH2:21][CH2:22][O:23][CH2:24][CH2:25]1.O=[C:19](O)[CH2:18][CH2:17][CH2:16]/[CH:15]=[C:14]1/[CH2:13][C@@H:12]2[C@@H:11](/[CH:10]=[CH:9]/[C@H:7]([CH:5]([CH2:4][C:3]#[C:2][CH3:1])[CH3:6])[OH:8])[C@H:29]([OH:30])[CH2:28][C@@H:27]2[CH2:26]1>>[CH3:1][C:2]#[C:3][CH2:4][CH:5]([CH3:6])[C@H:7]([OH:8])/[CH:9]=[CH:10]/[C@...
C1COCCN1.CC#CCC(C)[C@H](O)/C=C/[C@@H]1[C@H]2C/C(=C/CCCC(=O)O)C[C@H]2C[C@H]1O
CC#CCC(C)[C@H](O)/C=C/[C@@H]1[C@H]2C/C(=C/CCCCN3CCOCC3)C[C@H]2C[C@H]1O
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
OtherReaction
c60b8c5e8ed4f8735a6d92335f9d058f7ab0d9365e1bd9f6b6322ce378b11144
5fb52ddc67e52a472f28d69e60f3ac94989e70b5307ac3fa95fe53e87c1d2696
C(\CCCCN1CCOCC1)=C1\C[C@H]2CCC[C@H]2C1
O-[C;H0;D3;+0:1](=O)-[C:2]-[C:3].[#8:4]1-[C:5]-[C:6]-[NH;D2;+0:7]-[C:8]-[C:9]-1>>[C:3]-[C:2]-[CH2;D2;+0:1]-[N;H0;D3;+0:7]1-[C:6]-[C:5]-[#8:4]-[C:9]-[C:8]-1
40
[{"value": 40.0, "product": "O1CCN(CC1)CCCC\\C=C\\1/C[C@H]2C[C@H]([C@@H]([C@H]2C1)\\C=C\\[C@H](C(CC#CC)C)O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 30.4, "product": "O1CCN(CC1)CCCC\\C=C\\1/C[C@H]2C[C@H]([C@@H]([C@H]2C1)\\C=C\\[C@H](C(CC#CC)C)O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired":...
50
CELSIUS
1.5
HOUR
20 mg of (1S,2R,3R,5S)-7-[(E)-4-carboxybutylidene]-2-[(3S,1E)-3-hydroxy-4-methyl-6-octyne-1-enyl]-3-hydroxybicyclo[3.3.0]octane was taken and dissolved in 2 mL of dimethylformamide. After addition of 20 mg of 1,1′-carbonyldiimidazole, it was stirred at 50° C. for 1.5 hours. It was then cooled to ambient temperature, an...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amine
C1COCCN1
C1COCC[NH]1
C1C[C@H]2CCC[C@H]2C1.C1COCC[NH]1
Other
CN(C=O)C
50
1.5
C1COCCN1.CC#CCC(C)[C@H](O)/C=C/[C@@H]1[C@H]2C/C(=C/CCCC(=O)O)C[C@H]2C[C@H]1O>CN(C=O)C>CC#CCC(C)[C@H](O)/C=C/[C@@H]1[C@H]2C/C(=C/CCCCN3CCOCC3)C[C@H]2C[C@H]1O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a4f667ad199b4df4a69d9ad291606bb7
C1COCCN1.CC#CCC(C)[C@H](O)/C=C/[C@@H]1[C@H]2c3cccc(CCCC(=O)O)c3O[C@H]2C[C@H]1O>>CC#CCC(C)[C@H](O)/C=C/[C@@H]1[C@H]2c3cccc(CCCCN4CCOCC4)c3O[C@H]2C[C@H]1O
[Cl-].[NH4+].O[C@H]1[C@@H]([C@@H]2[C@@H](OC3=C2C=CC=C3CCCC(=O)O)C1)\C=C\[C@H](C(CC#CC)C)O.C(=O)(N1C=NC=C1)N1C=NC=C1.N1CCOCC1>>O[C@H]1[C@@H]([C@@H]2[C@@H](OC3=C2C=CC=C3CCCCN3CCOCC3)C1)\C=C\[C@H](C(CC#CC)C)O
[NH:22]1[CH2:23][CH2:24][O:25][CH2:26][CH2:27]1.O=[C:21](O)[CH2:20][CH2:19][CH2:18][c:17]1[cH:16][cH:15][cH:14][c:13]2[c:28]1[O:29][C@@H:30]1[C@H:12]2[C@@H:11](/[CH:10]=[CH:9]/[C@H:7]([CH:5]([CH2:4][C:3]#[C:2][CH3:1])[CH3:6])[OH:8])[C@H:32]([OH:33])[CH2:31]1>>[CH3:1][C:2]#[C:3][CH2:4][CH:5]([CH3:6])[C@H:7]([OH:8])/[CH:...
C1COCCN1.CC#CCC(C)[C@H](O)/C=C/[C@@H]1[C@H]2c3cccc(CCCC(=O)O)c3O[C@H]2C[C@H]1O
CC#CCC(C)[C@H](O)/C=C/[C@@H]1[C@H]2c3cccc(CCCCN4CCOCC4)c3O[C@H]2C[C@H]1O
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
OtherReaction
c60b8c5e8ed4f8735a6d92335f9d058f7ab0d9365e1bd9f6b6322ce378b11144
5fb52ddc67e52a472f28d69e60f3ac94989e70b5307ac3fa95fe53e87c1d2696
c1cc(CCCCN2CCOCC2)c2c(c1)[C@@H]1CCC[C@@H]1O2
O-[C;H0;D3;+0:1](=O)-[C:2]-[C:3].[#8:4]1-[C:5]-[C:6]-[NH;D2;+0:7]-[C:8]-[C:9]-1>>[C:3]-[C:2]-[CH2;D2;+0:1]-[N;H0;D3;+0:7]1-[C:6]-[C:5]-[#8:4]-[C:9]-[C:8]-1
48
[{"value": 48.0, "product": "O[C@H]1[C@@H]([C@@H]2[C@@H](OC3=C2C=CC=C3CCCCN3CCOCC3)C1)\\C=C\\[C@H](C(CC#CC)C)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 46.6, "product": "O[C@H]1[C@@H]([C@@H]2[C@@H](OC3=C2C=CC=C3CCCCN3CCOCC3)C1)\\C=C\\[C@H](C(CC#CC)C)O", "details": "CALCULATEDPERCENTYIELD", "is_desir...
50
CELSIUS
1
HOUR
10 mg of (1R,2R,3aS,8bS)-2,3,3a,8b-tetrahydro-2-hydroxy-1-[(3S,1E)-3-hydroxy-4-methyl-1-octene-6-ynyl]-5-(3-carboxypropyl)-1H-cyclopenta[b]benzofuran was taken and was dissolved in 2 mL of dimethylformamide. After addition of 8.1 mg of 1,1′-carbonyldiimidazole, it was stirred at 50° C. for 1 hour. It was cooled to ambi...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amine
C1COCCN1
C1COCC[NH]1
C1COCC[NH]1.c1ccc2c(c1)O[C@H]1CCC[C@@H]21
Other
CN(C=O)C
50
1
C1COCCN1.CC#CCC(C)[C@H](O)/C=C/[C@@H]1[C@H]2c3cccc(CCCC(=O)O)c3O[C@H]2C[C@H]1O>CN(C=O)C>CC#CCC(C)[C@H](O)/C=C/[C@@H]1[C@H]2c3cccc(CCCCN4CCOCC4)c3O[C@H]2C[C@H]1O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-af70023515324f95bea882d743822d1c
CI.Cc1cc(Br)ccc1N>>CNc1ccc(Br)cc1C
BrC1=CC(=C(N)C=C1)C.C(=O)([O-])[O-].[K+].[K+].IC>>CNC1=C(C=C(C=C1)Br)C
I[CH3:1].[NH2:2][c:3]1[cH:4][cH:5][c:6]([Br:7])[cH:8][c:9]1[CH3:10]>>[CH3:1][NH:2][c:3]1[cH:4][cH:5][c:6]([Br:7])[cH:8][c:9]1[CH3:10]
CI.Cc1cc(Br)ccc1N
CNc1ccc(Br)cc1C
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
N-alkylation of primary amines with alkyl halides
3c2788b3f372b76c1d2ee0d77963cb247b210aa8a28e76637b4e731826c4252a
c6874c6af41d3b1c4f7668e1cd342c90252d0e77f4317d31b3193ebc2f9501a3
c1ccccc1
I-[CH3;D1;+0:1].[NH2;D1;+0:2]-[c:3](:[c:4]):[c:5]>>[CH3;D1;+0:1]-[NH;D2;+0:2]-[c:3](:[c:4]):[c:5]
null
[]
null
null
14
HOUR
To a solution of 2.03 g (10.91 mmol) of 4-bromo-2-methylaniline in 40 ml of DMF was added 2.07 g (14.98 mmol) of K2CO3 and 0.63 ml (10.12 mmol) of iodomethane, and the mixture was stirred at room temperature for 14 hours. After this time, the reaction mixture was quenched by the addition of a saturated aqueous solution...
10.6084/m9.figshare.5104873.v1
null
Primary amine
Secondary amine
null
null
c1ccccc1
HI
CN(C)C=O
null
14
CI.Cc1cc(Br)ccc1N>CN(C)C=O>CNc1ccc(Br)cc1C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c7de15a5b80d4d3ca1aea6c4a4e5da0b
CNc1ccc(Br)cc1C.COc1ccc(CCl)cc1>>COc1ccc(CN(C)c2ccc(Br)cc2C)cc1
COC1=CC=C(CCl)C=C1.CNC1=C(C=C(C=C1)Br)C.[H-].[Na+]>>CN(C1=C(C=C(C=C1)Br)C)CC1=CC=C(C=C1)OC
[NH:8]([CH3:9])[c:10]1[cH:11][cH:12][c:13]([Br:14])[cH:15][c:16]1[CH3:17].Cl[CH2:7][c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:19][cH:18]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][N:8]([CH3:9])[c:10]2[cH:11][cH:12][c:13]([Br:14])[cH:15][c:16]2[CH3:17])[cH:18][cH:19]1
CNc1ccc(Br)cc1C.COc1ccc(CCl)cc1
COc1ccc(CN(C)c2ccc(Br)cc2C)cc1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
6d58cac08ccced0a33ed16fbca180bc12aa011288d6476106d98a7b2cbc3d709
523d37155b42c8dc851abeddadebb241cdd90bdf649ba750c35e13c8c752d7b0
c1ccc(CNc2ccccc2)cc1
Cl-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[C;D1;H3:5]-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]>>[C;D1;H3:5]-[N;H0;D3;+0:6](-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4])-[c:7](:[c:8]):[c:9]
null
[]
null
null
0.5
HOUR
To a solution of 2.7 g (13.57 mmol) of N-methyl-4-bromo-2-methylaniline in 20 ml of DMF at room temperature was added 608 mg (15.2 mmol) of NaH and the mixture was stirred at room temperature for 0.5 h. After this time, 2.05 ml (15.1 mmol) of 4-methoxybenzyl chloride was added and the reaction mixture was heated to 60°...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amine
Tertiary amine
null
null
c1ccccc1.c1ccccc1
HCl
CN(C)C=O
null
0.5
CNc1ccc(Br)cc1C.COc1ccc(CCl)cc1>CN(C)C=O>COc1ccc(CN(C)c2ccc(Br)cc2C)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-41d4930a785649b8835252e9e1c4c3e2
Cc1cc(Br)ccc1N(C)S(=O)(=O)c1ccccc1.O=C(c1ccccc1)C(F)(F)F>>CNc1ccc(C(O)(c2ccccc2)C(F)(F)F)cc1C
C(=O)(C(F)(F)F)O.FC(C(=O)C1=CC=CC=C1)(F)F.BrC1=CC(=C(C=C1)N(S(=O)(=O)C1=CC=CC=C1)C)C.[Li]C(C)(C)C>>FC(C(O)(C1=CC=CC=C1)C1=CC(=C(C=C1)NC)C)(F)F
O=S(=O)(c1ccccc1)[N:2]([CH3:1])[c:3]1[cH:4][cH:5][c:6](Br)[cH:19][c:20]1[CH3:21].[C:7](=[O:8])([c:9]1[cH:10][cH:11][cH:12][cH:13][cH:14]1)[C:15]([F:16])([F:17])[F:18]>>[CH3:1][NH:2][c:3]1[cH:4][cH:5][c:6]([C:7]([OH:8])([c:9]2[cH:10][cH:11][cH:12][cH:13][cH:14]2)[C:15]([F:16])([F:17])[F:18])[cH:19][c:20]1[CH3:21]
Cc1cc(Br)ccc1N(C)S(=O)(=O)c1ccccc1.O=C(c1ccccc1)C(F)(F)F
CNc1ccc(C(O)(c2ccccc2)C(F)(F)F)cc1C
null
null
C1CCOC1
C-C Coupling
OtherReaction
dede6ff79bd7f869797072aa63f73523791693b80f650aaa4ee655b252853c55
a54fb2b4a2d4c4f9e6988da61f3d85e6e8274065bcf7838ffd7a40da5a580474
c1ccc(Cc2ccccc2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](-[N;H0;D3;+0:5](-[C;D1;H3:6])-S(=O)(=O)-c2:c:c:c:c:c:2):[c:7]:[c:8]:1.[F;D1;H0:9]-[C:10](-[F;D1;H0:11])(-[F;D1;H0:12])-[C;H0;D3;+0:13](=[O;H0;D1;+0:14])-[c:15](:[c:16]):[c:17]>>[C;D1;H3:6]-[NH;D2;+0:5]-[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1](-[C;H0;D4;+0:13](-[OH;D1;+0:14])(-[c:15](:[c:16...
null
[]
-78
CELSIUS
0.5
HOUR
To a solution of 1.03 g (3.23 mmol) of N-(4-bromo-2-methylphenyl)-N-methyl-benzenesulfonamide in 30 ml THF at −78° C. was added dropwise 3.9 ml (6.63 mmol) of a 1.7M solution of tert-BuLi in hexanes and the resultant mixture was stirred at −78° C. for 0.5 h. To this mixture was then added 0.66 ml (4.7 mmol) of 2,2,2-tr...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ketone.Tertiary amine
Tertiary alcohol.Secondary amine
c1ccccc1.c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1
HBr
C1CCOC1
-78
0.5
Cc1cc(Br)ccc1N(C)S(=O)(=O)c1ccccc1.O=C(c1ccccc1)C(F)(F)F>C1CCOC1>CNc1ccc(C(O)(c2ccccc2)C(F)(F)F)cc1C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5753627b79654a82b0b98a7cd4b39a1f
CNc1ccc(C(O)(c2cccc(C(F)(F)F)c2)C(CF)(CF)CF)cc1C.O=S(=O)(Cl)c1ccccc1>>Cc1cc(C(O)(c2cccc(C(F)(F)F)c2)C(F)(F)F)ccc1N(C)S(=O)(=O)c1ccccc1
FCC(C(O)(C1=CC(=CC=C1)C(F)(F)F)C1=CC(=C(C=C1)NC)C)(CF)CF.C1(=CC=CC=C1)S(=O)(=O)Cl>>CN(S(=O)(=O)C1=CC=CC=C1)C1=C(C=C(C=C1)C(C(F)(F)F)(C1=CC(=CC=C1)C(F)(F)F)O)C
C([C:17](C[F:19])(C[F:20])[C:5]([c:4]1[cH:3][c:2]([CH3:1])[c:23]([NH:24][CH3:25])[cH:22][cH:21]1)([OH:6])[c:7]1[cH:8][cH:9][cH:10][c:11]([C:12]([F:13])([F:14])[F:15])[cH:16]1)[F:18].Cl[S:26](=[O:27])(=[O:28])[c:29]1[cH:30][cH:31][cH:32][cH:33][cH:34]1>>[CH3:1][c:2]1[cH:3][c:4]([C:5]([OH:6])([c:7]2[cH:8][cH:9][cH:10][c:...
CNc1ccc(C(O)(c2cccc(C(F)(F)F)c2)C(CF)(CF)CF)cc1C.O=S(=O)(Cl)c1ccccc1
Cc1cc(C(O)(c2cccc(C(F)(F)F)c2)C(F)(F)F)ccc1N(C)S(=O)(=O)c1ccccc1
null
null
null
Acylation
OtherReaction
123b2137a06084a4b3c1a6013c0cd92a1ec9938b1392d2a38e8a451464e6aa7c
0ac24d1a131e4ca9cf43f5228ce6ad99b7d350ee17451e901421de0c21e61ca4
O=S(=O)(Nc1ccc(Cc2ccccc2)cc1)c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[C;D1;H3:7]-[NH;D2;+0:8]-[c:9](:[c:10]):[c:11].[F;H0;D1;+0:12]-C-[C;H0;D4;+0:13](-C-[F;H0;D1;+0:14])(-C-[F;H0;D1;+0:15])-[C:16](-[O;D1;H1:17])(-[c:18])-[c:19]>>[C;D1;H3:7]-[N;H0;D3;+0:8](-[c:9](:[c:10]):[c:11])-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-...
null
[]
null
null
null
null
The title compound was prepared from 2,2,2-trifluoromethyl-1-(3-methyl-4-methylaminophenyl)-1-(3-trifluoromethyl-phenyl)-ethanol (Step A) and benzenesulfonyl chloride using the procedure described in Example 1, Step D. 1H-NMR (CDCl3) δ 2.41 (s, 3H), 3.15 (s, 3H), 6.64 (d, J=8.4 Hz, 1H), 7.18 (brs, 1H), 7.42 (brs, 1H), ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary halide.Primary halide.Secondary amine.Sulfonyl halide
Trifluoro group.Tertiary amine
null
null
c1ccccc1.c1ccccc1.c1ccccc1
HCl
null
null
null
CNc1ccc(C(O)(c2cccc(C(F)(F)F)c2)C(CF)(CF)CF)cc1C.O=S(=O)(Cl)c1ccccc1>>Cc1cc(C(O)(c2cccc(C(F)(F)F)c2)C(F)(F)F)ccc1N(C)S(=O)(=O)c1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-56c612ddbb804f2eaca1a9a515e8f4cf
CN(c1ccc(C(=O)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1.Clc1cc[c]([Mg][Br])cc1>>CN(c1ccc(C(O)(c2ccc(Cl)cc2)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1
CN(S(=O)(=O)C1=CC=CC=C1)C1=CC=C(C=C1)C(C(F)(F)F)=O.ClC1=CC=C(C=C1)[Mg]Br>>ClC1=CC=C(C=C1)C(C(F)(F)F)(O)C1=CC=C(C=C1)N(S(=O)(=O)C1=CC=CC=C1)C
[CH3:1][N:2]([c:3]1[cH:4][cH:5][c:6]([C:7](=[O:8])[C:16]([F:17])([F:18])[F:19])[cH:20][cH:21]1)[S:22](=[O:23])(=[O:24])[c:25]1[cH:26][cH:27][cH:28][cH:29][cH:30]1.[Br][Mg][c:9]1[cH:10][cH:11][c:12]([Cl:13])[cH:14][cH:15]1>>[CH3:1][N:2]([c:3]1[cH:4][cH:5][c:6]([C:7]([OH:8])([c:9]2[cH:10][cH:11][c:12]([Cl:13])[cH:14][cH:...
CN(c1ccc(C(=O)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1.Clc1cc[c]([Mg][Br])cc1
CN(c1ccc(C(O)(c2ccc(Cl)cc2)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1
null
null
C1CCOC1
C-C Coupling
Grignard from ketone to alcohol
181fdd58eba73242b2de454099edbf422e18f2a0a3f78d67208494cf1d83905c
5854166cd4ea706bc07d74dc79eb8f4a990bc6c5eacbf0ca947d88ee86e78fdf
O=S(=O)(Nc1ccc(Cc2ccccc2)cc1)c1ccccc1
[Br]-[Mg]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[F;D1;H0:6]-[C:7](-[F;D1;H0:8])(-[F;D1;H0:9])-[C;H0;D3;+0:10](=[O;H0;D1;+0:11])-[c:12](:[c:13]):[c:14]>>[F;D1;H0:6]-[C:7](-[F;D1;H0:8])(-[F;D1;H0:9])-[C;H0;D4;+0:10](-[OH;D1;+0:11])(-[c:12](:[c:13]):[c:14])-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
null
[]
-78
CELSIUS
4
HOUR
To a solution of 0.2 g of N-methyl-N-(4-trifluoroacetyl-phenyl)-benzenesulfonamide in 10 mL of THF were added 0.7 mL of a 1M solution 4-chlorophenyl magnesium bromide at −78° C. The resulting mixture was stirred at −78° C. for 4 hr. After this time, the reaction mixture was quenched by the addition of a saturated aqueo...
10.6084/m9.figshare.5104873.v1
null
Magnesium halide.Ketone
Tertiary alcohol
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1.c1ccccc1
Br-.Mg
C1CCOC1
-78
4
CN(c1ccc(C(=O)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1.Clc1cc[c]([Mg][Br])cc1>C1CCOC1>CN(c1ccc(C(O)(c2ccc(Cl)cc2)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-068cd57809ed447eb08a6bef3d7309e1
CN(c1ccc(C(=O)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1.COCn1ccnc1>>COCn1ccnc1C(O)(c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
CN(S(=O)(=O)C1=CC=CC=C1)C1=CC=C(C=C1)C(C(F)(F)F)=O.COCN1C=NC=C1.C(CCC)[Li]>>CN(S(=O)(=O)C1=CC=CC=C1)C1=CC=C(C=C1)C(C(F)(F)F)(C=1N(C=CN1)COC)O
[C:9](=[O:10])([c:11]1[cH:12][cH:13][c:14]([N:15]([CH3:16])[S:17](=[O:18])(=[O:19])[c:20]2[cH:21][cH:22][cH:23][cH:24][cH:25]2)[cH:26][cH:27]1)[C:28]([F:29])([F:30])[F:31].[CH3:1][O:2][CH2:3][n:4]1[cH:5][cH:6][n:7][cH:8]1>>[CH3:1][O:2][CH2:3][n:4]1[cH:5][cH:6][n:7][c:8]1[C:9]([OH:10])([c:11]1[cH:12][cH:13][c:14]([N:15]...
CN(c1ccc(C(=O)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1.COCn1ccnc1
COCn1ccnc1C(O)(c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
null
null
C1CCOC1
C-C Coupling
OtherReaction
6437c5442b1284778f29095577cfe2e46b8a5b4ae4a931f781e1b4367639985a
454f67ba8644982dc9f605915a0f36178771eadaffb50d3f1e0f17f2b6fdeb10
O=S(=O)(Nc1ccc(Cc2ncc[nH]2)cc1)c1ccccc1
[C:1]-[#7;a:2]1:[c:3]:[c:4]:[#7;a:5]:[cH;D2;+0:6]:1.[F;D1;H0:7]-[C:8](-[F;D1;H0:9])(-[F;D1;H0:10])-[C;H0;D3;+0:11](=[O;H0;D1;+0:12])-[c:13](:[c:14]):[c:15]>>[C:1]-[#7;a:2]1:[c:3]:[c:4]:[#7;a:5]:[c;H0;D3;+0:6]:1-[C;H0;D4;+0:11](-[OH;D1;+0:12])(-[c:13](:[c:14]):[c:15])-[C:8](-[F;D1;H0:7])(-[F;D1;H0:9])-[F;D1;H0:10]
null
[]
null
null
14
HOUR
To a solution of 55 mg (0.49 mmol) of 1-methoxymethyl-1H-imidazole in 5 ml of THF at −78° C. was added 0.20 ml (0.50 mmol) of a 2.5 M solution of n-butyllithium in hexanes and the resultant mixture was stirred at −78° C. for 30 mins. After this time, a solution of 160 mg (0.47 mmol) of N-methyl-N-(4-trifluoroacetyl-phe...
10.6084/m9.figshare.5104873.v1
null
Ketone
Tertiary alcohol
c1c[nH]cn1
c1ncc[nH]1
c1ncc[nH]1.c1ccccc1.c1ccccc1
null
C1CCOC1
null
14
CN(c1ccc(C(=O)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1.COCn1ccnc1>C1CCOC1>COCn1ccnc1C(O)(c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-272692371c074155b8e4bdc7870a2a38
C#Cc1ccccc1.CN(c1ccc(C(=O)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1>>CN(c1ccc(C(O)(C#Cc2ccccc2)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1
CN(S(=O)(=O)C1=CC=CC=C1)C1=CC=C(C=C1)C(C(F)(F)F)=O.C1(=CC=CC=C1)C#C.[Li]CCCC>>OC(C#CC1=CC=CC=C1)(C(F)(F)F)C1=CC=C(C=C1)N(S(=O)(=O)C1=CC=CC=C1)C
[CH:9]#[C:10][c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1.[CH3:1][N:2]([c:3]1[cH:4][cH:5][c:6]([C:7](=[O:8])[C:17]([F:18])([F:19])[F:20])[cH:21][cH:22]1)[S:23](=[O:24])(=[O:25])[c:26]1[cH:27][cH:28][cH:29][cH:30][cH:31]1>>[CH3:1][N:2]([c:3]1[cH:4][cH:5][c:6]([C:7]([OH:8])([C:9]#[C:10][c:11]2[cH:12][cH:13][cH:14][cH:15][...
C#Cc1ccccc1.CN(c1ccc(C(=O)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1
CN(c1ccc(C(O)(C#Cc2ccccc2)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1
null
null
C1CCOC1
C-C Coupling
OtherReaction
2ddb79a55c34731f669ca9c81c37bd79ca03c4be0b8aa443046efbe4fb65f2a7
77853d31b4fad0a859afba1c4b23a275023e810d45fe8d791ab91aae7d1b14c5
O=S(=O)(Nc1ccc(CC#Cc2ccccc2)cc1)c1ccccc1
[CH;D1;+0:1]#[C:2]-[c:3].[F;D1;H0:4]-[C:5](-[F;D1;H0:6])(-[F;D1;H0:7])-[C;H0;D3;+0:8](=[O;H0;D1;+0:9])-[c:10](:[c:11]):[c:12]>>[F;D1;H0:4]-[C:5](-[F;D1;H0:6])(-[F;D1;H0:7])-[C;H0;D4;+0:8](-[OH;D1;+0:9])(-[C;H0;D2;+0:1]#[C:2]-[c:3])-[c:10](:[c:11]):[c:12]
null
[]
-78
CELSIUS
30
MINUTE
To a solution of 0.18 g of phenylacetylene (1.75 mmol) in 5 mL of THF was added dropwise 0.76 mL of n-BuLi (2.5M in hexane) at −78° C. The color of the solution turned dark blue and the mixture was stirred at −78° C. for 30 min. Then 0.5 g of N-methyl-N-(4-trifluoroacetyl-phenyl)-benzenesulfonamide (Example 22, Step A)...
10.6084/m9.figshare.5104873.v1
null
Ketone.Alkyne
Tertiary alcohol.Alkyne
null
null
c1ccccc1.c1ccccc1.c1ccccc1
null
C1CCOC1
-78
0.5
C#Cc1ccccc1.CN(c1ccc(C(=O)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1>C1CCOC1>CN(c1ccc(C(O)(C#Cc2ccccc2)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-9173a36377bb49c8a9885055e531babe
C#CC(F)(F)F.CN(c1ccc(C(=O)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1>>CN(c1ccc(C(O)(C#CC(F)(F)F)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1
CN(S(=O)(=O)C1=CC=CC=C1)C1=CC=C(C=C1)C(C(F)(F)F)=O.FC(C#C)(F)F>>CN(S(=O)(=O)C1=CC=CC=C1)C1=CC=C(C=C1)C(C#CC(F)(F)F)(C(F)(F)F)O
[CH:9]#[C:10][C:11]([F:12])([F:13])[F:14].[CH3:1][N:2]([c:3]1[cH:4][cH:5][c:6]([C:7](=[O:8])[C:15]([F:16])([F:17])[F:18])[cH:19][cH:20]1)[S:21](=[O:22])(=[O:23])[c:24]1[cH:25][cH:26][cH:27][cH:28][cH:29]1>>[CH3:1][N:2]([c:3]1[cH:4][cH:5][c:6]([C:7]([OH:8])([C:9]#[C:10][C:11]([F:12])([F:13])[F:14])[C:15]([F:16])([F:17])...
C#CC(F)(F)F.CN(c1ccc(C(=O)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1
CN(c1ccc(C(O)(C#CC(F)(F)F)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1
null
null
null
C-C Coupling
OtherReaction
2ddb79a55c34731f669ca9c81c37bd79ca03c4be0b8aa443046efbe4fb65f2a7
77853d31b4fad0a859afba1c4b23a275023e810d45fe8d791ab91aae7d1b14c5
O=S(=O)(Nc1ccccc1)c1ccccc1
[CH;D1;+0:1]#[C:2]-[C:3](-[F;D1;H0:4])(-[F;D1;H0:5])-[F;D1;H0:6].[F;D1;H0:7]-[C:8](-[F;D1;H0:9])(-[F;D1;H0:10])-[C;H0;D3;+0:11](=[O;H0;D1;+0:12])-[c:13](:[c:14]):[c:15]>>[F;D1;H0:4]-[C:3](-[F;D1;H0:5])(-[F;D1;H0:6])-[C:2]#[C;H0;D2;+0:1]-[C;H0;D4;+0:11](-[OH;D1;+0:12])(-[c:13](:[c:14]):[c:15])-[C:8](-[F;D1;H0:7])(-[F;D1...
null
[]
null
null
null
null
The compound was prepared from N-methyl-N-(4-trifluoroacetyl-phenyl)-benzenesulfonamide (Example 22, Step A) and 3,3,3-trifluoroprop-1-yne following the procedure described in Example 29. 1H NMR (CDCl3) δ 3.19 (s, 3H), 4.30 (br s, 1H), 7.11–7.63 (m, 9H). Mass Spectrum (CI+) m/e=438 (M+1). Conditions: See reaction.notes...
10.6084/m9.figshare.5104873.v1
null
Ketone.Alkyne
Tertiary alcohol.Alkyne
null
null
c1ccccc1.c1ccccc1
null
null
null
null
C#CC(F)(F)F.CN(c1ccc(C(=O)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1>>CN(c1ccc(C(O)(C#CC(F)(F)F)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-86d8cb05cde84ed19ba311853bb41f4b
C#CCC(C)C.CN(c1ccc(C(=O)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1>>CC(C)CC#CC(O)(c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
CN(S(=O)(=O)C1=CC=CC=C1)C1=CC=C(C=C1)C(C(F)(F)F)=O.CC(CC#C)C>>OC(C#CCC(C)C)(C(F)(F)F)C1=CC=C(C=C1)N(S(=O)(=O)C1=CC=CC=C1)C
[CH3:1][CH:2]([CH3:3])[CH2:4][C:5]#[CH:6].[C:7](=[O:8])([c:9]1[cH:10][cH:11][c:12]([N:13]([CH3:14])[S:15](=[O:16])(=[O:17])[c:18]2[cH:19][cH:20][cH:21][cH:22][cH:23]2)[cH:24][cH:25]1)[C:26]([F:27])([F:28])[F:29]>>[CH3:1][CH:2]([CH3:3])[CH2:4][C:5]#[C:6][C:7]([OH:8])([c:9]1[cH:10][cH:11][c:12]([N:13]([CH3:14])[S:15](=[O...
C#CCC(C)C.CN(c1ccc(C(=O)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1
CC(C)CC#CC(O)(c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
null
null
null
C-C Coupling
OtherReaction
2ddb79a55c34731f669ca9c81c37bd79ca03c4be0b8aa443046efbe4fb65f2a7
77853d31b4fad0a859afba1c4b23a275023e810d45fe8d791ab91aae7d1b14c5
O=S(=O)(Nc1ccccc1)c1ccccc1
[C:1]-[C:2]#[CH;D1;+0:3].[F;D1;H0:4]-[C:5](-[F;D1;H0:6])(-[F;D1;H0:7])-[C;H0;D3;+0:8](=[O;H0;D1;+0:9])-[c:10](:[c:11]):[c:12]>>[C:1]-[C:2]#[C;H0;D2;+0:3]-[C;H0;D4;+0:8](-[OH;D1;+0:9])(-[c:10](:[c:11]):[c:12])-[C:5](-[F;D1;H0:4])(-[F;D1;H0:6])-[F;D1;H0:7]
null
[]
null
null
null
null
The compound was prepared from N-methyl-N-(4-trifluoroacetyl-phenyl)-benzenesulfonamide (Example 22, Step A) and 4-methyl-pent-1-yne following the procedure described in Example 29. 1H NMR (CDCl3) δ 1.01 (d, J=6.6 Hz, 6H), 1.90 (sept, J=6.6 Hz, 1H), 2.21 (d, J=7.7 Hz, 2H), 3.17 (s, 3H), 3.24 (br s, 1H), 7.12–7.68 (m, 9...
10.6084/m9.figshare.5104873.v1
null
Ketone.Alkyne
Tertiary alcohol.Alkyne
null
null
c1ccccc1.c1ccccc1
null
null
null
null
C#CCC(C)C.CN(c1ccc(C(=O)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1>>CC(C)CC#CC(O)(c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-2a2989db33d445c4b96af396a0efd1b0
NC1CCCC1.O=C(c1ccc(F)cc1)C(F)(F)F>>O=C(c1ccc(NC2CCCC2)cc1)C(F)(F)F
FC(C(=O)C1=CC=C(C=C1)F)(F)F.C(C)N(CC)CC.C1(CCCC1)N>>C1(CCCC1)NC1=CC=C(C=C1)C(C(F)(F)F)=O
[NH2:7][CH:8]1[CH2:9][CH2:10][CH2:11][CH2:12]1.F[c:6]1[cH:5][cH:4][c:3]([C:2](=[O:1])[C:15]([F:16])([F:17])[F:18])[cH:14][cH:13]1>>[O:1]=[C:2]([c:3]1[cH:4][cH:5][c:6]([NH:7][CH:8]2[CH2:9][CH2:10][CH2:11][CH2:12]2)[cH:13][cH:14]1)[C:15]([F:16])([F:17])[F:18]
NC1CCCC1.O=C(c1ccc(F)cc1)C(F)(F)F
O=C(c1ccc(NC2CCCC2)cc1)C(F)(F)F
null
null
C(C)#N
Heteroatom Alkylation and Arylation
Buchwald-Hartwig/Ullmann-Goldberg/N-arylation primary amine
da9dae6a655c4bd18887b692f91621e77027436294d6e1fc7be7295afb364796
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1ccc(NC2CCCC2)cc1
F-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[C:6]-[C:7](-[NH2;D1;+0:8])-[C:9]>>[C:6]-[C:7](-[NH;D2;+0:8]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5])-[C:9]
null
[]
null
null
null
null
To a mixture of 3.94 g of 2,2,2,4′-tetrafluoroacetophenone (20.5 mmol) and 3.35 ml triethylamine (24.0 mmol) in 40 ml of acetonitrile at 0° C. were added 5.9 ml of cyclopentylamine (59.8 mmol). The reaction was allowed to warm to room temperature and then heated to reflux for 14 h. After this time the reaction mixture ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ccccc1
c1ccccc1
c1ccccc1.C1CCCC1
HF
C(C)#N
null
null
NC1CCCC1.O=C(c1ccc(F)cc1)C(F)(F)F>C(C)#N>O=C(c1ccc(NC2CCCC2)cc1)C(F)(F)F
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-905bcbd6cf02468cae9f1104f7cb26a1
C#Cc1ccccc1.O=C(c1ccc(NC2CCCC2)cc1)C(F)(F)F>>OC(C#Cc1ccccc1)(c1ccc(NC2CCCC2)cc1)C(F)(F)F
C1(CCCC1)NC1=CC=C(C=C1)C(C(F)(F)F)=O.C1(=CC=CC=C1)C#C.C(CCC)[Li]>>C1(CCCC1)NC1=CC=C(C=C1)C(C(F)(F)F)(C#CC1=CC=CC=C1)O
[CH:3]#[C:4][c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1.[O:1]=[C:2]([c:11]1[cH:12][cH:13][c:14]([NH:15][CH:16]2[CH2:17][CH2:18][CH2:19][CH2:20]2)[cH:21][cH:22]1)[C:23]([F:24])([F:25])[F:26]>>[OH:1][C:2]([C:3]#[C:4][c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1)([c:11]1[cH:12][cH:13][c:14]([NH:15][CH:16]2[CH2:17][CH2:18][CH2:19][CH2...
C#Cc1ccccc1.O=C(c1ccc(NC2CCCC2)cc1)C(F)(F)F
OC(C#Cc1ccccc1)(c1ccc(NC2CCCC2)cc1)C(F)(F)F
null
null
C1CCOC1
C-C Coupling
OtherReaction
2ddb79a55c34731f669ca9c81c37bd79ca03c4be0b8aa443046efbe4fb65f2a7
77853d31b4fad0a859afba1c4b23a275023e810d45fe8d791ab91aae7d1b14c5
C(#Cc1ccccc1)Cc1ccc(NC2CCCC2)cc1
[CH;D1;+0:1]#[C:2]-[c:3].[F;D1;H0:4]-[C:5](-[F;D1;H0:6])(-[F;D1;H0:7])-[C;H0;D3;+0:8](=[O;H0;D1;+0:9])-[c:10](:[c:11]):[c:12]>>[F;D1;H0:4]-[C:5](-[F;D1;H0:6])(-[F;D1;H0:7])-[C;H0;D4;+0:8](-[OH;D1;+0:9])(-[C;H0;D2;+0:1]#[C:2]-[c:3])-[c:10](:[c:11]):[c:12]
null
[]
-78
CELSIUS
30
MINUTE
To a solution of 0.4 ml of phenylacetylene (3.6 mmol in 10 ml of THF at −78° C. was added 1.9 ml (4.75 mmol) of a 2.5 M solution of n-butyllithium in hexanes. The color of the solution turned dark blue and the reaction mixture was stirred at −78° C. for 30 min. After this time, a solution of 450 mg of 1-(4-cyclopentyla...
10.6084/m9.figshare.5104873.v1
null
Ketone.Alkyne
Tertiary alcohol.Alkyne
null
null
c1ccccc1.c1ccccc1.C1CCCC1
null
C1CCOC1
-78
0.5
C#Cc1ccccc1.O=C(c1ccc(NC2CCCC2)cc1)C(F)(F)F>C1CCOC1>OC(C#Cc1ccccc1)(c1ccc(NC2CCCC2)cc1)C(F)(F)F
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a44c26cf9d6443bda601b2b6b77d0b6c
O=S(=O)(Cl)c1cc(Cl)ccc1Cl.OC(C#Cc1ccccc1)(c1ccc(NC2CCCC2)cc1)C(F)(F)F>>O=S(=O)(c1cc(Cl)ccc1Cl)N(c1ccc(C(O)(C#Cc2ccccc2)C(F)(F)F)cc1)C1CCCC1
C1(CCCC1)NC1=CC=C(C=C1)C(C(F)(F)F)(C#CC1=CC=CC=C1)O.ClC1=C(C=C(C=C1)Cl)S(=O)(=O)Cl>>ClC1=C(C=C(C=C1)Cl)S(=O)(=O)N(C1=CC=C(C=C1)C(C#CC1=CC=CC=C1)(C(F)(F)F)O)C1CCCC1
Cl[S:2](=[O:1])(=[O:3])[c:4]1[cH:5][c:6]([Cl:7])[cH:8][cH:9][c:10]1[Cl:11].[NH:12]([c:13]1[cH:14][cH:15][c:16]([C:17]([OH:18])([C:19]#[C:20][c:21]2[cH:22][cH:23][cH:24][cH:25][cH:26]2)[C:27]([F:28])([F:29])[F:30])[cH:31][cH:32]1)[CH:33]1[CH2:34][CH2:35][CH2:36][CH2:37]1>>[O:1]=[S:2](=[O:3])([c:4]1[cH:5][c:6]([Cl:7])[cH...
O=S(=O)(Cl)c1cc(Cl)ccc1Cl.OC(C#Cc1ccccc1)(c1ccc(NC2CCCC2)cc1)C(F)(F)F
O=S(=O)(c1cc(Cl)ccc1Cl)N(c1ccc(C(O)(C#Cc2ccccc2)C(F)(F)F)cc1)C1CCCC1
null
null
N1=CC=CC=C1
Acylation
Sulfonamide synthesis (Schotten-Baumann) secondary amine
abeb6d9a0c70fe5baef0a8e555c2cd55ac2317f763ce7a0831775db7a04777d8
b7aca5a5d690b0846685a854bc946849e1041bfc3965161290b5ffb2821af09e
O=S(=O)(c1ccccc1)N(c1ccc(CC#Cc2ccccc2)cc1)C1CCCC1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[C:7]-[C:8](-[NH;D2;+0:9]-[c:10](:[c:11]):[c:12])-[C:13]>>[C:7]-[C:8](-[N;H0;D3;+0:9](-[c:10](:[c:11]):[c:12])-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6])-[C:13]
null
[]
70
CELSIUS
null
null
A mixture of 53 mg of 2-(4-cyclopentylamino-phenyl)-1,1,1-trifluoro-4-phenyl-but-3-yn-2-ol (0.15 mmol) and 44 mg of 2,5-dichlorobenzenesulfonyl chloride (0.18 mmol) in 0.2 ml of pyridine was heated to 70° C. for 14 hours. After this time the reaction mixture was allowed to cool to room temperature, quenched by the addi...
10.6084/m9.figshare.5104873.v1
null
Secondary amine.Sulfonyl halide
Tertiary amine
null
null
c1ccccc1.c1ccccc1.c1ccccc1.C1CCCC1
HCl
N1=CC=CC=C1
70
null
O=S(=O)(Cl)c1cc(Cl)ccc1Cl.OC(C#Cc1ccccc1)(c1ccc(NC2CCCC2)cc1)C(F)(F)F>N1=CC=CC=C1>O=S(=O)(c1cc(Cl)ccc1Cl)N(c1ccc(C(O)(C#Cc2ccccc2)C(F)(F)F)cc1)C1CCCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ab4cba9ad83843d2a764bfbec7274330
CC(C)CN.O=S(=O)(Cl)c1ccccc1>>CC(C)CNS(=O)(=O)c1ccccc1
C(C(C)C)N.C(C)N(CC)CC.C1(=CC=CC=C1)S(=O)(=O)Cl>>C(C(C)C)NS(=O)(=O)C1=CC=CC=C1
[CH3:1][CH:2]([CH3:3])[CH2:4][NH2:5].Cl[S:6](=[O:7])(=[O:8])[c:9]1[cH:10][cH:11][cH:12][cH:13][cH:14]1>>[CH3:1][CH:2]([CH3:3])[CH2:4][NH:5][S:6](=[O:7])(=[O:8])[c:9]1[cH:10][cH:11][cH:12][cH:13][cH:14]1
CC(C)CN.O=S(=O)(Cl)c1ccccc1
CC(C)CNS(=O)(=O)c1ccccc1
null
null
C(Cl)Cl
Miscellaneous
Sulfonamide synthesis (Schotten-Baumann) primary amine
a86b0632821e188c0a5dc5a5a2aac298ab3eccaee8a52ba46078c3d5975a290d
50f8fbf3d327483c3eeff8f6cbd4065e4c7600bb501fbe08958a5c79a0926428
c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[C:7]-[C:8]-[NH2;D1;+0:9]>>[C:7]-[C:8]-[NH;D2;+0:9]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]
null
[]
0
CELSIUS
30
MINUTE
To a solution of 4.14 g of isobutylamine (56.6 mmol) and 2.86 g of triethylamine (28.3 mmol) in 40 mL of CH2Cl2 was slowly added 5.0 g of benzenesulfonyl chloride (28.3 mmol) at 0° C. The resulting mixture was stirred at 0° C. for 30 min and then at rt for 1 hr. 150 mL of CH2Cl2 were added, and the organic layer was wa...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccccc1
HCl
C(Cl)Cl
0
0.5
CC(C)CN.O=S(=O)(Cl)c1ccccc1>C(Cl)Cl>CC(C)CNS(=O)(=O)c1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c3bc4ba7f6bb4a54a7d11f396736f8e8
CC(C)CN(c1ccc(C(O)(C#CC(=O)O)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1.CN>>CNC(=O)C#CC(O)(c1ccc(N(CC(C)C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
C1(=CC=CC=C1)S(=O)(=O)N(C1=CC=C(C=C1)C(C#CC(=O)O)(C(F)(F)F)O)CC(C)C.CN.Cl.CN(CCCN=C=NCC)C>>CNC(C#CC(C(F)(F)F)(O)C1=CC=C(C=C1)N(CC(C)C)S(=O)(=O)C1=CC=CC=C1)=O
O[C:3](=[O:4])[C:5]#[C:6][C:7]([OH:8])([c:9]1[cH:10][cH:11][c:12]([N:13]([CH2:14][CH:15]([CH3:16])[CH3:17])[S:18](=[O:19])(=[O:20])[c:21]2[cH:22][cH:23][cH:24][cH:25][cH:26]2)[cH:27][cH:28]1)[C:29]([F:30])([F:31])[F:32].[CH3:1][NH2:2]>>[CH3:1][NH:2][C:3](=[O:4])[C:5]#[C:6][C:7]([OH:8])([c:9]1[cH:10][cH:11][c:12]([N:13]...
CC(C)CN(c1ccc(C(O)(C#CC(=O)O)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1.CN
CNC(=O)C#CC(O)(c1ccc(N(CC(C)C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
null
null
C(Cl)Cl
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=S(=O)(Nc1ccccc1)c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]#[C:4]-[C:5].[C;D1;H3:6]-[NH2;D1;+0:7]>>[C:5]-[C:4]#[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:7]-[C;D1;H3:6]
null
[]
null
null
16
HOUR
0.2 g of 4-[4-(benzenesulfonyl-isobutyl-amino)-phenyl]-5,5,5-trifluoro-4-hydroxy-pent-2-ynoic acid (see Example 69; 0.439 mmol) and 0.26 mL of methylamine (2M in THF) were combined in 3 mL of CH2Cl2 at rt. 0.1 g of 1-[3-(dimethylamino)propyl]-3-ethylcarbodiimide hydrochloride (0.527 mmol) was added. The resulting mixtu...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccccc1
HO-
C(Cl)Cl
null
16
CC(C)CN(c1ccc(C(O)(C#CC(=O)O)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1.CN>C(Cl)Cl>CNC(=O)C#CC(O)(c1ccc(N(CC(C)C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-68c1b2678fec4a839319799f6101cb08
CC(C)CN(c1ccc(C(O)(C#C[Si](C)(C)C)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1>>C#CC(O)(c1ccc(N(CC(C)C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
OC(C#C[Si](C)(C)C)(C(F)(F)F)C1=CC=C(C=C1)N(S(=O)(=O)C1=CC=CC=C1)CC(C)C.[F-].C(CCC)[N+](CCCC)(CCCC)CCCC>>OC(C#C)(C(F)(F)F)C1=CC=C(C=C1)N(S(=O)(=O)C1=CC=CC=C1)CC(C)C
C[Si](C)(C)[C:1]#[C:2][C:3]([OH:4])([c:5]1[cH:6][cH:7][c:8]([N:9]([CH2:10][CH:11]([CH3:12])[CH3:13])[S:14](=[O:15])(=[O:16])[c:17]2[cH:18][cH:19][cH:20][cH:21][cH:22]2)[cH:23][cH:24]1)[C:25]([F:26])([F:27])[F:28]>>[CH:1]#[C:2][C:3]([OH:4])([c:5]1[cH:6][cH:7][c:8]([N:9]([CH2:10][CH:11]([CH3:12])[CH3:13])[S:14](=[O:15])(...
CC(C)CN(c1ccc(C(O)(C#C[Si](C)(C)C)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1
C#CC(O)(c1ccc(N(CC(C)C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
null
null
C(Cl)Cl.C1CCOC1
Deprotection
TMS deprotection from alkyne
e85676bb81da384790c9c858d44f182cdd01e3a79f77f7a239fe38487234cb96
56d526d7c9cb1bd7bee4940e216a9b1dd4597fd025a186b8d6e4675d8f4db26b
O=S(=O)(Nc1ccccc1)c1ccccc1
C-[Si](-C)(-C)-[C;H0;D2;+0:1]#[C:2]-[C:3]>>[C:3]-[C:2]#[CH;D1;+0:1]
null
[]
null
null
1
HOUR
To a solution of 0.25 g (0.51 mmol) of N-[4-(1-hydroxy-1-trifluoromethyl-3-trimethylsilanyl-prop-2-ynyl)-phenyl]-N-isobutyl-benzenesulfonamide (Example 74) in 6 mL of CH2Cl2 was added 0.4 mL of a 1 M solution of tetrabutylammonium fluoride in THF. The mixture was stirred at room temperature for 1 hour. CH2Cl2 (60 mL) w...
10.6084/m9.figshare.5104873.v1
null
Alkyne.Silyl protective group
Alkyne
null
null
c1ccccc1.c1ccccc1
Other
C(Cl)Cl.C1CCOC1
null
1
CC(C)CN(c1ccc(C(O)(C#C[Si](C)(C)C)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1>C(Cl)Cl.C1CCOC1>C#CC(O)(c1ccc(N(CC(C)C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4b6978f8aa5c4493b9190309ea64498e
Brc1ccc2ccccc2c1.C#CC(O)(c1ccc(N(CC(C)C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F>>CC(C)CN(c1ccc(C(O)(C#Cc2cccc3ccccc23)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1
BrC1=CC2=CC=CC=C2C=C1.O.C(=O)([O-])[O-].[K+].[K+].OC(C#C)(C(F)(F)F)C1=CC=C(C=C1)N(S(=O)(=O)C1=CC=CC=C1)CC(C)C>>OC(C#CC1=CC=CC2=CC=CC=C12)(C(F)(F)F)C1=CC=C(C=C1)N(S(=O)(=O)C1=CC=CC=C1)CC(C)C
Br[c:15]1[cH:14][c:23]2[c:18]([cH:17][cH:16]1)[cH:19][cH:20][cH:21][cH:22]2.[CH3:1][CH:2]([CH3:3])[CH2:4][N:5]([c:6]1[cH:7][cH:8][c:9]([C:10]([OH:11])([C:12]#[CH:13])[C:24]([F:25])([F:26])[F:27])[cH:28][cH:29]1)[S:30](=[O:31])(=[O:32])[c:33]1[cH:34][cH:35][cH:36][cH:37][cH:38]1>>[CH3:1][CH:2]([CH3:3])[CH2:4][N:5]([c:6]...
Brc1ccc2ccccc2c1.C#CC(O)(c1ccc(N(CC(C)C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
CC(C)CN(c1ccc(C(O)(C#Cc2cccc3ccccc23)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1
null
[Pd].[Cu]I
COCCOC
C-C Coupling
OtherReaction
427d52803b094b22f8f109b6c17c82e6ccc9792ebeaad9bc5ad19cad543470b3
305eca0fd2975da49e7f69e4edfb9dc1cbce82513954bc5a73be3289e70e5f76
O=S(=O)(Nc1ccc(CC#Cc2cccc3ccccc23)cc1)c1ccccc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[c:5](:[c:6]):[cH;D2;+0:7]:1.[C:8]-[C:9]#[CH;D1;+0:10]>>[C:8]-[C:9]#[C;H0;D2;+0:10]-[c;H0;D3;+0:7]1:[cH;D2;+0:1]:[c:2]:[c:3]:[c:4]:[c:5]:1:[c:6]
null
[]
null
null
30
MINUTE
80.6 mg (0.39 mmol) 2-Bromonaphthalene, 21 mg palladium on carbon (10% Pd), 74.1 mg (0.39 mmol) copper (I) iodide, and 135 mg (0.98 mmol) K2CO3 were combined 2 mL of DME and 2 mL of water and the resulting mixture was stirred at room temperature for 30 min. A solution of 80 mg (0.2 mmol) of N-[4-(1-hydroxy-1-trifluorom...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Alkyne
Alkyne
c1ccc2ccccc2c1
c1ccc2ccccc2c1
c1ccccc1.c1ccc2ccccc2c1.c1ccccc1
HBr
[Pd].[Cu]I.COCCOC
null
0.5
Brc1ccc2ccccc2c1.C#CC(O)(c1ccc(N(CC(C)C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F>[Pd].[Cu]I.COCCOC>CC(C)CN(c1ccc(C(O)(C#Cc2cccc3ccccc23)C(F)(F)F)cc1)S(=O)(=O)c1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c9e8b955dadb4be390e459aed7fa1256
CCOCCBr.O=C(c1ccc[nH]1)C(F)(F)F>>CCOCCn1cccc1C(=O)C(F)(F)F
[H-].[Na+].FC(C(=O)C=1NC=CC1)(F)F.C(C)OCCBr>>C(C)OCCN1C(=CC=C1)C(C(F)(F)F)=O
Br[CH2:5][CH2:4][O:3][CH2:2][CH3:1].[nH:6]1[cH:7][cH:8][cH:9][c:10]1[C:11](=[O:12])[C:13]([F:14])([F:15])[F:16]>>[CH3:1][CH2:2][O:3][CH2:4][CH2:5][n:6]1[cH:7][cH:8][cH:9][c:10]1[C:11](=[O:12])[C:13]([F:14])([F:15])[F:16]
CCOCCBr.O=C(c1ccc[nH]1)C(F)(F)F
CCOCCn1cccc1C(=O)C(F)(F)F
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
161a14961e9f1b305dfb4891994ad58540b58501680f8eb4ba76ad15e1e7cb96
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1cc[nH]c1
Br-[CH2;D2;+0:1]-[C:2]-[#8:3].[F;D1;H0:4]-[C:5](-[F;D1;H0:6])(-[F;D1;H0:7])-[C:8](=[O;D1;H0:9])-[c:10]1:[c:11]:[c:12]:[c:13]:[nH;D2;+0:14]:1>>[#8:3]-[C:2]-[CH2;D2;+0:1]-[n;H0;D3;+0:14]1:[c:13]:[c:12]:[c:11]:[c:10]:1-[C:8](=[O;D1;H0:9])-[C:5](-[F;D1;H0:4])(-[F;D1;H0:6])-[F;D1;H0:7]
null
[]
0
CELSIUS
1
HOUR
To a suspension of 268 mg (6.70 mmol) of NaH (60% dispersion in oil) in 20 mL DMF at 0° C. was added 1.01 g (6.19 mmol) of 2-(trifluoroacteyl)pyrrole and the mixture was stirred at 0° C. for 1 h. After this time, 765 μL (6.51 mmol) of 2-bromoethyl ethyl ether was added and the mixture was warmed to 60° C. and stirred f...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1cc[nH]c1
c1ccc[nH]1
c1ccc[nH]1
HBr
CN(C)C=O
0
1
CCOCCBr.O=C(c1ccc[nH]1)C(F)(F)F>CN(C)C=O>CCOCCn1cccc1C(=O)C(F)(F)F
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d1e33565cabe49e5b2004b2758236b11
CNc1ccc(Br)cc1.O=S(=O)(Cl)c1ccccc1>>CN(c1ccc(Br)cc1)S(=O)(=O)c1ccccc1
BrC1=CC=C(NC)C=C1.C1(=CC=CC=C1)S(=O)(=O)Cl>>BrC1=CC=C(C=C1)N(S(=O)(=O)C1=CC=CC=C1)C
[CH3:1][NH:2][c:3]1[cH:4][cH:5][c:6]([Br:7])[cH:8][cH:9]1.Cl[S:10](=[O:11])(=[O:12])[c:13]1[cH:14][cH:15][cH:16][cH:17][cH:18]1>>[CH3:1][N:2]([c:3]1[cH:4][cH:5][c:6]([Br:7])[cH:8][cH:9]1)[S:10](=[O:11])(=[O:12])[c:13]1[cH:14][cH:15][cH:16][cH:17][cH:18]1
CNc1ccc(Br)cc1.O=S(=O)(Cl)c1ccccc1
CN(c1ccc(Br)cc1)S(=O)(=O)c1ccccc1
null
null
N1=CC=CC=C1
Miscellaneous
Sulfonamide synthesis (Schotten-Baumann) secondary amine
f885e88ea942f3030166da4c7f20dfb8bf6f1e152c7507d56458611df7dc3120
971e620478d668662a3bf915b510f5704d42a595d6ca9c67de007bd5d7063a75
O=S(=O)(Nc1ccccc1)c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[C;D1;H3:7]-[NH;D2;+0:8]-[c:9](:[c:10]):[c:11]>>[C;D1;H3:7]-[N;H0;D3;+0:8](-[c:9](:[c:10]):[c:11])-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]
null
[]
null
null
null
null
A solution of 0.61 g (3.3 mmol) of 4-bromo-N-methylaniline and 0.5 mL (3.92 mmol) of benzenesulfonyl chloride in 5 mL of pyridine was stirred for 12 h at rt. After that time the pyridine was removed by azeotropic distillation with heptane. The residue was purified by chromatography on silica (hexanes:EtOAc, 9:1) to giv...
10.6084/m9.figshare.5104873.v1
null
Secondary amine.Sulfonyl halide
Tertiary amine
null
null
c1ccccc1.c1ccccc1
HCl
N1=CC=CC=C1
null
null
CNc1ccc(Br)cc1.O=S(=O)(Cl)c1ccccc1>N1=CC=CC=C1>CN(c1ccc(Br)cc1)S(=O)(=O)c1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-cbf5c4679a00474b8f5f7f699350d347
CCOCCn1cccc1C(=O)C(F)(F)F.CN(c1ccc(Br)cc1)S(=O)(=O)c1ccccc1>>CCOCCn1cccc1C(O)(c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
C(C)OCCN1C(=CC=C1)C(C(F)(F)F)=O.BrC1=CC=C(C=C1)N(S(=O)(=O)C1=CC=CC=C1)C.[Li]C(C)(C)C>>C(C)OCCN1C(=CC=C1)C(C(F)(F)F)(O)C1=CC=C(C=C1)N(S(=O)(=O)C1=CC=CC=C1)C
[CH3:1][CH2:2][O:3][CH2:4][CH2:5][n:6]1[cH:7][cH:8][cH:9][c:10]1[C:11](=[O:12])[C:30]([F:31])([F:32])[F:33].Br[c:13]1[cH:14][cH:15][c:16]([N:17]([CH3:18])[S:19](=[O:20])(=[O:21])[c:22]2[cH:23][cH:24][cH:25][cH:26][cH:27]2)[cH:28][cH:29]1>>[CH3:1][CH2:2][O:3][CH2:4][CH2:5][n:6]1[cH:7][cH:8][cH:9][c:10]1[C:11]([OH:12])([...
CCOCCn1cccc1C(=O)C(F)(F)F.CN(c1ccc(Br)cc1)S(=O)(=O)c1ccccc1
CCOCCn1cccc1C(O)(c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
null
null
CCOCC.CCCCC.C1CCOC1
C-C Coupling
Grignard_alcohol
23831eb2f5100c758a065f977b2daac4728a2009a2a7f37e9b01c50283e9e583
b8801be51258f6ee39fb6aad45dd9677b1b9eed3d6e0018ffb065bca8e787abf
O=S(=O)(Nc1ccc(Cc2ccc[nH]2)cc1)c1ccccc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[C:6]-[#7;a:7](:[c:8]):[c:9](-[C;H0;D3;+0:10](=[O;H0;D1;+0:11])-[C:12](-[F;D1;H0:13])(-[F;D1;H0:14])-[F;D1;H0:15]):[c:16]>>[C:6]-[#7;a:7](:[c:8]):[c:9](-[C;H0;D4;+0:10](-[OH;D1;+0:11])(-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5])-[C:12](-[F;D1;H0:13])(-[F;D1;H0:14])-[F;D1;H0:15...
null
[]
null
null
null
null
To a solution of 75 mg (0.23 mmol) of N-(4-bromophenyl)-N-methyl-benzenesulfonamide in 4 mL of Et2O at −78° C. was added dropwise 285 μL (0.49 mmol) of a 1.7 M solution of tert-BuLi in pentane and the resultant mixture was stirred at −78° C. for 10 min. To this mixture was then added a solution of 81 mg (0.34 mmol) of ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ketone
Tertiary alcohol
c1ccccc1
c1ccccc1
c1ccc[nH]1.c1ccccc1.c1ccccc1
Br-
CCOCC.CCCCC.C1CCOC1
null
null
CCOCCn1cccc1C(=O)C(F)(F)F.CN(c1ccc(Br)cc1)S(=O)(=O)c1ccccc1>CCOCC.CCCCC.C1CCOC1>CCOCCn1cccc1C(O)(c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5ae3e8692b2f4f589d0a29c32af72885
CI.COCCn1cccc1C(O)(c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F>>COCCn1cccc1C(OC)(c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
[H-].[Na+].COCCN1C(=CC=C1)C(C(F)(F)F)(O)C1=CC=C(C=C1)N(S(=O)(=O)C1=CC=CC=C1)C.IC>>COCCN1C(=CC=C1)C(C(F)(F)F)(OC)C1=CC=C(C=C1)N(S(=O)(=O)C1=CC=CC=C1)C
I[CH3:12].[CH3:1][O:2][CH2:3][CH2:4][n:5]1[cH:6][cH:7][cH:8][c:9]1[C:10]([OH:11])([c:13]1[cH:14][cH:15][c:16]([N:17]([CH3:18])[S:19](=[O:20])(=[O:21])[c:22]2[cH:23][cH:24][cH:25][cH:26][cH:27]2)[cH:28][cH:29]1)[C:30]([F:31])([F:32])[F:33]>>[CH3:1][O:2][CH2:3][CH2:4][n:5]1[cH:6][cH:7][cH:8][c:9]1[C:10]([O:11][CH3:12])([...
CI.COCCn1cccc1C(O)(c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
COCCn1cccc1C(OC)(c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
cd10a9010f842ab825b304bd2965f17f9c39c4c64e5fc6cd91306ae51817de0d
9271b713ded6954f3329c61a211042ac37c82b3aff1b62cb455035e69339dd27
O=S(=O)(Nc1ccc(Cc2ccc[nH]2)cc1)c1ccccc1
I-[CH3;D1;+0:1].[#7;a:2]:[c:3]-[C:4](-[OH;D1;+0:5])(-[c:6])-[C:7](-[F;D1;H0:8])(-[F;D1;H0:9])-[F;D1;H0:10]>>[#7;a:2]:[c:3]-[C:4](-[c:6])(-[O;H0;D2;+0:5]-[CH3;D1;+0:1])-[C:7](-[F;D1;H0:8])(-[F;D1;H0:9])-[F;D1;H0:10]
null
[]
0
CELSIUS
35
MINUTE
To a suspension of 3.8 mg of NaH (0.10 mmol) in 3 mL of DMF at 0° C. was added 32 mg of N-(4-{-[1-(2-methoxyethyl)-1H-pyrrol-2-yl]-2,2,2-trifluoro-1-hydroxyethyl}-phenyl)-N-methyl-benzenesulfonamide (Example 79, 0.068 mmol) and the reaction mixture was stirred at 0° C. for 35 min. 6 μL of iodomethane (0.089 mmol) was a...
10.6084/m9.figshare.5104873.v1
null
Tertiary alcohol
Ether
null
null
c1ccc[nH]1.c1ccccc1.c1ccccc1
HI
CN(C)C=O
0
0.583333
CI.COCCn1cccc1C(O)(c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F>CN(C)C=O>COCCn1cccc1C(OC)(c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-8c4550540a824d66b849dd341f27b37d
CCOCCn1cccc1C(O)(c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F>>CCOCCn1cccc1C(c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
B(F)(F)F.CCOCC.C(C)OCCN1C(=CC=C1)C(C(F)(F)F)(O)C1=CC=C(C=C1)N(S(=O)(=O)C1=CC=CC=C1)C.C(C)[SiH](CC)CC>>C(C)OCCN1C(=CC=C1)C(C(F)(F)F)C1=CC=C(C=C1)N(S(=O)(=O)C1=CC=CC=C1)C
O[C:11]([c:10]1[n:6]([CH2:5][CH2:4][O:3][CH2:2][CH3:1])[cH:7][cH:8][cH:9]1)([c:12]1[cH:13][cH:14][c:15]([N:16]([CH3:17])[S:18](=[O:19])(=[O:20])[c:21]2[cH:22][cH:23][cH:24][cH:25][cH:26]2)[cH:27][cH:28]1)[C:29]([F:30])([F:31])[F:32]>>[CH3:1][CH2:2][O:3][CH2:4][CH2:5][n:6]1[cH:7][cH:8][cH:9][c:10]1[CH:11]([c:12]1[cH:13]...
CCOCCn1cccc1C(O)(c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
CCOCCn1cccc1C(c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
null
null
C(Cl)Cl
Reduction
OtherReaction
c74e766e62dea6513290ab98d06521c92685074430a200193315f473ed0037ec
dfa71f841ee148297c95b5d95b7150768ab9356304fca8dbfde20c6dadd639d3
O=S(=O)(Nc1ccc(Cc2ccc[nH]2)cc1)c1ccccc1
O-[C;H0;D4;+0:1](-[c:2](:[c:3]):[#7;a:4](-[C:5]):[c:6])(-[c:7](:[c:8]):[c:9])-[C:10](-[F;D1;H0:11])(-[F;D1;H0:12])-[F;D1;H0:13]>>[C:5]-[#7;a:4](:[c:6]):[c:2](-[CH;D3;+0:1](-[c:7](:[c:8]):[c:9])-[C:10](-[F;D1;H0:11])(-[F;D1;H0:12])-[F;D1;H0:13]):[c:3]
null
[]
null
null
1.75
HOUR
To a solution of 32 mg (0.07 mmol) of N-(4-{1-[1-(2-ethoxyethyl)-1H-pyrrol-2-yl]-2,2,2-trifluoro-1-hydroxyethyl}-phenyl)-N-methyl-benzenesulfonamide (Example 78) in 2 mL of CH2Cl2 at 0° C. were added 1.05 mL (6.57 mmol) of triethylsilane followed by 167 μL (1.32 mmol) of boron trifluoride diethyl etherate dropwise. The...
10.6084/m9.figshare.5104873.v1
null
Tertiary alcohol
null
null
null
c1ccc[nH]1.c1ccccc1.c1ccccc1
Other
C(Cl)Cl
null
1.75
CCOCCn1cccc1C(O)(c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F>C(Cl)Cl>CCOCCn1cccc1C(c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1)C(F)(F)F
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-32943dafa0ec4be9a66701c171835240
CN(c1ccc(Br)cc1)S(=O)(=O)c1ccccc1.COCCn1cccc1C=O>>COCCn1cccc1C(O)c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1
COCCN1C(=CC=C1)C=O.BrC1=CC=C(C=C1)N(S(=O)(=O)C1=CC=CC=C1)C.[Li]C(C)(C)C>>OC(C=1N(C=CC1)CCOC)C1=CC=C(C=C1)N(S(=O)(=O)C1=CC=CC=C1)C
Br[c:12]1[cH:13][cH:14][c:15]([N:16]([CH3:17])[S:18](=[O:19])(=[O:20])[c:21]2[cH:22][cH:23][cH:24][cH:25][cH:26]2)[cH:27][cH:28]1.[CH3:1][O:2][CH2:3][CH2:4][n:5]1[cH:6][cH:7][cH:8][c:9]1[CH:10]=[O:11]>>[CH3:1][O:2][CH2:3][CH2:4][n:5]1[cH:6][cH:7][cH:8][c:9]1[CH:10]([OH:11])[c:12]1[cH:13][cH:14][c:15]([N:16]([CH3:17])[S...
CN(c1ccc(Br)cc1)S(=O)(=O)c1ccccc1.COCCn1cccc1C=O
COCCn1cccc1C(O)c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1
null
null
CCCCC.C1CCOC1
C-C Coupling
Grignard_alcohol
0c8bc0f755f4d9a2cfce93ae43a9a9a531fa8ad86ff120aed0a18ba03c84e4d7
1c0bd0afc1d5e370e3c8193faf738f03752295e40fa0eb99c756011e9a4be26b
O=S(=O)(Nc1ccc(Cc2ccc[nH]2)cc1)c1ccccc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].[C:6]-[#7;a:7](:[c:8]):[c:9](-[CH;D2;+0:10]=[O;H0;D1;+0:11]):[c:12]>>[C:6]-[#7;a:7](:[c:8]):[c:9](-[CH;D3;+0:10](-[OH;D1;+0:11])-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:12]
null
[]
-30
CELSIUS
null
null
To a solution of 1.49 g (4.59 mmol) of N-(4-bromophenyl)-N-methyl benzenesulfonamide (Example 78, Step C) in 37.5 mL THF at −78° C. was added dropwise 5.94 mL (10.10 mmol) of a 1.7 M solution of tert-BuLi in pentane and the resultant mixture was stirred at −78° C. for 15 min. To this mixture was then added a solution o...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aldehyde
Secondary alcohol
c1ccccc1
c1ccccc1
c1ccc[nH]1.c1ccccc1.c1ccccc1
Br-
CCCCC.C1CCOC1
-30
null
CN(c1ccc(Br)cc1)S(=O)(=O)c1ccccc1.COCCn1cccc1C=O>CCCCC.C1CCOC1>COCCn1cccc1C(O)c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5de3c28587d841a49d898ee79598a074
COCCn1cccc1C(O)c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1>>COCCn1cccc1Cc1ccc(N(C)S(=O)(=O)c2ccccc2)cc1
B(F)(F)F.CCOCC.OC(C=1N(C=CC1)CCOC)C1=CC=C(C=C1)N(S(=O)(=O)C1=CC=CC=C1)C.C(C)[SiH](CC)CC>>COCCN1C(=CC=C1)CC1=CC=C(C=C1)N(S(=O)(=O)C1=CC=CC=C1)C
O[CH:10]([c:9]1[n:5]([CH2:4][CH2:3][O:2][CH3:1])[cH:6][cH:7][cH:8]1)[c:11]1[cH:12][cH:13][c:14]([N:15]([CH3:16])[S:17](=[O:18])(=[O:19])[c:20]2[cH:21][cH:22][cH:23][cH:24][cH:25]2)[cH:26][cH:27]1>>[CH3:1][O:2][CH2:3][CH2:4][n:5]1[cH:6][cH:7][cH:8][c:9]1[CH2:10][c:11]1[cH:12][cH:13][c:14]([N:15]([CH3:16])[S:17](=[O:18])...
COCCn1cccc1C(O)c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1
COCCn1cccc1Cc1ccc(N(C)S(=O)(=O)c2ccccc2)cc1
null
null
C(Cl)Cl
Reduction
OtherReaction
3c5af32aa639db2ebe4d9851942e9468e1838e06ae5b2c1669bca1d5e0922c33
46f8a11b80b06e754a5a34198d843342612a5e7ede950bda52ce3a500cedba0b
O=S(=O)(Nc1ccc(Cc2ccc[nH]2)cc1)c1ccccc1
O-[CH;D3;+0:1](-[c:2](:[c:3]):[c:4])-[c:5](:[c:6]):[#7;a:7](-[C:8]):[c:9]>>[C:8]-[#7;a:7](:[c:9]):[c:5](-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]):[c:6]
null
[]
null
null
2.5
HOUR
To a solution of 16 mg (0.04 mmol) of N-(4-{1-hydroxy-1-[1-(2-methoxyethyl)-1H-pyrrol-2-yl]-methyl}-phenyl)-N-methyl-benzenesulfonamide (Example 93) in 1.5 mL CH2Cl2 at 0° C. were added 620 μL (3.88 mmol) of triethylsilane followed by 100 μL (0.79 mmol) of boron trifluoride diethyl etherate dropwise. The mixture was wa...
10.6084/m9.figshare.5104873.v1
null
Secondary alcohol
null
null
null
c1ccc[nH]1.c1ccccc1.c1ccccc1
Other
C(Cl)Cl
null
2.5
COCCn1cccc1C(O)c1ccc(N(C)S(=O)(=O)c2ccccc2)cc1>C(Cl)Cl>COCCn1cccc1Cc1ccc(N(C)S(=O)(=O)c2ccccc2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-57535bf7c107433c9e25a290b71400a3
C=C(CCl)CCl.CC(=O)c1ccc(O)c(CS(=O)(=O)c2ccccc2)c1>>C=C(CCl)COc1ccc(C(=O)OC)cc1CS(=O)(=O)c1ccccc1
C([O-])([O-])=O.[K+].[K+].ClCC(=C)CCl.OC1=C(C=C(C=C1)C(C)=O)CS(=O)(=O)C1=CC=CC=C1.CN(C=O)C.Cl>>ClCC(COC1=C(C=C(C(=O)OC)C=C1)CS(=O)(=O)C1=CC=CC=C1)=C
Cl[CH2:5][C:2](=[CH2:1])[CH2:3][Cl:4].[OH:6][c:7]1[cH:8][cH:9][c:10]([C:11](=[O:12])[CH3:14])[cH:15][c:16]1[CH2:17][S:18](=[O:19])(=[O:20])[c:21]1[cH:22][cH:23][cH:24][cH:25][cH:26]1>>[CH2:1]=[C:2]([CH2:3][Cl:4])[CH2:5][O:6][c:7]1[cH:8][cH:9][c:10]([C:11](=[O:12])[O:13][CH3:14])[cH:15][c:16]1[CH2:17][S:18](=[O:19])(=[O...
C=C(CCl)CCl.CC(=O)c1ccc(O)c(CS(=O)(=O)c2ccccc2)c1
C=C(CCl)COc1ccc(C(=O)OC)cc1CS(=O)(=O)c1ccccc1
null
[I-].C(CCC)[N+](CCCC)(CCCC)CCCC
O.CCOCC
Acylation
OtherReaction
77178c9f76d901cb1fe6c7e159adafad906b7ae05c375169b03230411ae03429
4c394635b02fb0de5299b7d137e911f21c9ebfc0eec1816ad013f170ce0f9fe0
O=S(=O)(Cc1ccccc1)c1ccccc1
Cl-[CH2;D2;+0:1]-[C:2](-[C:3])=[C;D1;H2:4].[CH3;D1;+0:5]-[C;H0;D3;+0:6](=[O;D1;H0:7])-[c:8]1:[c:9]:[c:10]:[c:11](-[OH;D1;+0:12]):[c:13]:[c:14]:1>>[C:3]-[C:2](=[C;D1;H2:4])-[CH2;D2;+0:1]-[O;H0;D2;+0:12]-[c:11]1:[c:10]:[c:9]:[c:8](-[C;H0;D3;+0:6](=[O;D1;H0:7])-[#8:15]-[CH3;D1;+0:5]):[c:14]:[c:13]:1
50
[{"value": 50.0, "product": "ClCC(COC1=C(C=C(C(=O)OC)C=C1)CS(=O)(=O)C1=CC=CC=C1)=C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
20
HOUR
3 g (8.62 mmol) of tetrabutylammonium iodide, 3.02 g (20.4 mmol) of potassium carbonate and then 2.36 ml (20.4 mmol) of 2-chloromethyl-3-chloro-1-propene are successively introduced into a solution of 2.5 g (8.16 mmol) of readily accessible 1-{4-hydroxy-3-[(phenylsulfonyl)methyl]phenyl}ethanone in 150 ml of N,N-dimethy...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ketone.Aromatic alcohol
Ester.Ether
null
null
c1ccccc1.c1ccccc1
null
[I-].C(CCC)[N+](CCCC)(CCCC)CCCC.O.CCOCC
null
20
C=C(CCl)CCl.CC(=O)c1ccc(O)c(CS(=O)(=O)c2ccccc2)c1>[I-].C(CCC)[N+](CCCC)(CCCC)CCCC.O.CCOCC>C=C(CCl)COc1ccc(C(=O)OC)cc1CS(=O)(=O)c1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d1d71153d7a647bc86d1440342c2fac6
C=C(CCl)COc1ccc(C(=O)OC)cc1CS(=O)(=O)c1ccccc1>>C=C1COc2ccc(C(=O)OC)cc2C(S(=O)(=O)c2ccccc2)C1
O.Cl.C[Si](C)(C)[N-][Si](C)(C)C.[Li+].ClCC(COC1=C(C=C(C(=O)OC)C=C1)CS(=O)(=O)C1=CC=CC=C1)=C>>C=C1COC2=C(C(C1)S(=O)(=O)C1=CC=CC=C1)C=C(C=C2)C(=O)OC
Cl[CH2:25][C:2](=[CH2:1])[CH2:3][O:4][c:5]1[cH:6][cH:7][c:8]([C:9](=[O:10])[O:11][CH3:12])[cH:13][c:14]1[CH2:15][S:16](=[O:17])(=[O:18])[c:19]1[cH:20][cH:21][cH:22][cH:23][cH:24]1>>[CH2:1]=[C:2]1[CH2:3][O:4][c:5]2[cH:6][cH:7][c:8]([C:9](=[O:10])[O:11][CH3:12])[cH:13][c:14]2[CH:15]([S:16](=[O:17])(=[O:18])[c:19]2[cH:20]...
C=C(CCl)COc1ccc(C(=O)OC)cc1CS(=O)(=O)c1ccccc1
C=C1COc2ccc(C(=O)OC)cc2C(S(=O)(=O)c2ccccc2)C1
null
null
ClCCl.O1CCCC1
Functional Group Interconversion
OtherReaction
6b8c466c96c7381d3c662d12cbde5fb716a993369c63e8a3d9a4d09da309a087
47a659f5704a5b7ca1b92ff731f18f109c6bde1d45152a3a393eefbd10265508
C=C1COc2ccccc2C(S(=O)(=O)c2ccccc2)C1
Cl-[CH2;D2;+0:1]-[C:2](-[C:3])=[C;D1;H2:4].[O;D1;H0:5]=[#16:6](=[O;D1;H0:7])(-[c:8])-[CH2;D2;+0:9]-[c:10](:[c:11]):[c:12]>>[C:3]-[C:2](=[C;D1;H2:4])-[CH2;D2;+0:1]-[CH;D3;+0:9](-[#16:6](=[O;D1;H0:5])(=[O;D1;H0:7])-[c:8])-[c:10](:[c:11]):[c:12]
60
[{"value": 60.0, "product": "C=C1COC2=C(C(C1)S(=O)(=O)C1=CC=CC=C1)C=C(C=C2)C(=O)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 59.7, "product": "C=C1COC2=C(C(C1)S(=O)(=O)C1=CC=CC=C1)C=C(C=C2)C(=O)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
5
MINUTE
1.33 ml of 1.06M lithium bis(trimethylsilyl)amide in tetrahydrofuran are added to 478 mg (1.21 mmol) of methyl 4-{[2-(chloromethyl)-2-propenyl]oxy}-3-[(phenylsulfonyl)methyl]benzoate dissolved in 39 ml of tetrahydrofuran. The solution is stirred for 5 minutes and then water, 1N hydrochloric acid and dichloromethane are...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
null
c1ccc2c(c1)CCCCO2
c1ccc2c(c1)CCCCO2.c1ccccc1
HCl
ClCCl.O1CCCC1
null
0.083333
C=C(CCl)COc1ccc(C(=O)OC)cc1CS(=O)(=O)c1ccccc1>ClCCl.O1CCCC1>C=C1COc2ccc(C(=O)OC)cc2C(S(=O)(=O)c2ccccc2)C1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0688c3ac6a054939b48bf4505142ac19
C=C1COc2ccc(C(=O)OC)cc2C(S(=O)(=O)c2ccccc2)C1>>C=C1CCc2cc(C(=O)OC)ccc2OC1
C=C1COC2=C(C(C1)S(=O)(=O)C1=CC=CC=C1)C=C(C=C2)C(=O)OC.O.P(=O)(O)([O-])[O-].[Na+].[Na+].CO.O1CCCC1>>C=C1COC2=C(CC1)C=C(C=C2)C(=O)OC
O=S(=O)(c1ccccc1)[CH:4]1[CH2:3][C:2](=[CH2:1])[CH2:16][O:15][c:14]2[c:5]1[cH:6][c:7]([C:8](=[O:9])[O:10][CH3:11])[cH:12][cH:13]2>>[CH2:1]=[C:2]1[CH2:3][CH2:4][c:5]2[cH:6][c:7]([C:8](=[O:9])[O:10][CH3:11])[cH:12][cH:13][c:14]2[O:15][CH2:16]1
C=C1COc2ccc(C(=O)OC)cc2C(S(=O)(=O)c2ccccc2)C1
C=C1CCc2cc(C(=O)OC)ccc2OC1
null
[Na].[Hg]
ClCCl
Reduction
OtherReaction
1403cc7e5a2a911fded57203a36f53d3d03026d3cf24a05d673aa2af9b974752
d840e89f7e5c2afbebc71c3968f0da9c2e720c3c085dce57700b061c879e763d
C=C1CCc2ccccc2OC1
O=S(=O)(-[CH;D3;+0:1]1-[C:2]-[C:3](=[C;D1;H2:4])-[C:5]-[#8:6]-[c:7]:[c:8]-1:[c:9])-c1:c:c:c:c:c:1>>[C;D1;H2:4]=[C:3]1-[C:5]-[#8:6]-[c:7]:[c:8](:[c:9])-[CH2;D2;+0:1]-[C:2]-1
null
[]
null
null
4
HOUR
728 mg (0.95 mmol) of 3% sodium amalgam are added portionwise at 0° C. to a suspension of 85 mg (0.23 mmol) of methyl 3-methylene-5-(phenylsulfonyl)-2,3,4,5-tetrahydro-1-benzoxepin-7-carboxylate, prepared according to example 1, and of 116 mg (0.95 mmol) of sodium hydrogenphosphate in 10 ml of a 1/1 methanol/tetrahydro...
10.6084/m9.figshare.5104873.v1
null
Sulfone
null
c1ccccc1.c1ccc2c(c1)CCCCO2
c1ccc2c(c1)CCCCO2
c1ccc2c(c1)CCCCO2
HO-
[Na].[Hg].ClCCl
null
4
C=C1COc2ccc(C(=O)OC)cc2C(S(=O)(=O)c2ccccc2)C1>[Na].[Hg].ClCCl>C=C1CCc2cc(C(=O)OC)ccc2OC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d43c41bede90405fa3fc743006c413f3
COC(=O)c1ccc2c(c1)CCC(=O)CO2.ClC[P+](c1ccccc1)(c1ccccc1)c1ccccc1>>COC(=O)c1ccc2c(c1)CCC(=CCl)CO2
O=C1COC2=C(CC1)C=C(C=C2)C(=O)OC.C(CCC)[Li].[Cl-].ClC[P+](C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1.O>>ClC=C1COC2=C(CC1)C=C(C=C2)C(=O)OC
O=[C:13]1[CH2:12][CH2:11][c:9]2[c:8]([cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:10]2)[O:17][CH2:16]1.c1ccc([P+](c2ccccc2)(c2ccccc2)[CH2:14][Cl:15])cc1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]2[c:9]([cH:10]1)[CH2:11][CH2:12][C:13](=[CH:14][Cl:15])[CH2:16][O:17]2
COC(=O)c1ccc2c(c1)CCC(=O)CO2.ClC[P+](c1ccccc1)(c1ccccc1)c1ccccc1
COC(=O)c1ccc2c(c1)CCC(=CCl)CO2
null
null
O1CCCC1.CCCCCC
C-C Coupling
Wittig with Phosphonium
33f4b01bff17bc186870f174aa1415cc072a6904bf349e20bef59f70b19d9e13
4ccc953afa1928fe5ef55f22a0c593e017875730e9bc8868efb0bd3550ea5ba6
[CH]=C1CCc2ccccc2OC1
O=[C;H0;D3;+0:1](-[C:2]-[C:3])-[C:4]-[#8:5]-[c:6].[Cl;D1;H0:7]-[CH2;D2;+0:8]-[P+](-c1:c:c:c:c:c:1)(-c1:c:c:c:c:c:1)-c1:c:c:c:c:c:1>>[C:3]-[C:2]-[C;H0;D3;+0:1](=[CH;D2;+0:8]-[Cl;D1;H0:7])-[C:4]-[#8:5]-[c:6]
24.2
[{"value": 24.0, "product": "ClC=C1COC2=C(CC1)C=C(C=C2)C(=O)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 24.2, "product": "ClC=C1COC2=C(CC1)C=C(C=C2)C(=O)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
1
HOUR
0.08 ml (0.2 mmol) of a 1.9M solution of n-butyllithium in hexane is added dropwise to a suspension of 76 mg (0.22 mmol) of chloromethyltriphenylphosphonium chloride in 1.7 ml of tetrahydrofuran cooled to 0° C. The solution is stirred for one hour and then 40 mg (0.18 mmol) of methyl 3-oxo-2,3,4,5-tetrahydro-1-benzoxep...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ketone
null
c1ccc2c(c1)CCCCO2.c1ccccc1.c1ccccc1.c1ccccc1
c1ccc2c(c1)CCCCO2
c1ccc2c(c1)CCCCO2
HO-
O1CCCC1.CCCCCC
0
1
COC(=O)c1ccc2c(c1)CCC(=O)CO2.ClC[P+](c1ccccc1)(c1ccccc1)c1ccccc1>O1CCCC1.CCCCCC>COC(=O)c1ccc2c(c1)CCC(=CCl)CO2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-8e1a81dcc4f34c74882563a072dc0774
BrCc1ccccc1.C=C1COc2ccc(C(=O)OC)cc2C(S(=O)(=O)c2ccccc2)C1>>C=C1COc2ccc(C(=O)OC)cc2C(Cc2ccccc2)(S(=O)(=O)c2ccccc2)C1
C(C1=CC=CC=C1)Br.Cl.CN1C(N(CCC1)C)=O.C[Si](C)(C)[N-][Si](C)(C)C.[Li+].C=C1COC2=C(C(C1)S(=O)(=O)C1=CC=CC=C1)C=C(C=C2)C(=O)OC>>C(C1=CC=CC=C1)C1(CC(COC2=C1C=C(C=C2)C(=O)OC)=C)S(=O)(=O)C2=CC=CC=C2
Br[CH2:16][c:17]1[cH:18][cH:19][cH:20][cH:21][cH:22]1.[CH2:1]=[C:2]1[CH2:3][O:4][c:5]2[cH:6][cH:7][c:8]([C:9](=[O:10])[O:11][CH3:12])[cH:13][c:14]2[CH:15]([S:23](=[O:24])(=[O:25])[c:26]2[cH:27][cH:28][cH:29][cH:30][cH:31]2)[CH2:32]1>>[CH2:1]=[C:2]1[CH2:3][O:4][c:5]2[cH:6][cH:7][c:8]([C:9](=[O:10])[O:11][CH3:12])[cH:13]...
BrCc1ccccc1.C=C1COc2ccc(C(=O)OC)cc2C(S(=O)(=O)c2ccccc2)C1
C=C1COc2ccc(C(=O)OC)cc2C(Cc2ccccc2)(S(=O)(=O)c2ccccc2)C1
null
null
O1CCCC1.O.ClCCl
C-C Coupling
OtherReaction
0a2d11efff7a4620e79514433af23ac3b11c4e0755c270119fc4a9c5add176d9
f5e5e22797736d188bba28deb76a4cee8e4fee4dca04fe24f733d2ee68a23361
C=C1COc2ccccc2C(Cc2ccccc2)(S(=O)(=O)c2ccccc2)C1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[C;D1;H2:5]=[C:6]1-[C:7]-[CH;D3;+0:8](-[#16:9](=[O;D1;H0:10])(=[O;D1;H0:11])-[c:12])-[c:13](:[c:14]):[c:15]-[#8:16]-[C:17]-1>>[C;D1;H2:5]=[C:6]1-[C:7]-[C;H0;D4;+0:8](-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4])(-[#16:9](=[O;D1;H0:10])(=[O;D1;H0:11])-[c:12])-[c:13](:[c:14]):[c:15]-[#8:16]-[C:...
86
[{"value": 86.0, "product": "C(C1=CC=CC=C1)C1(CC(COC2=C1C=C(C=C2)C(=O)OC)=C)S(=O)(=O)C2=CC=CC=C2", "details": "PERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
0.072 ml (1.1 equivalents) of 1,3-dimethyl-3,4,5,6-tetrahydro-2(1H)-pyrimidinone and then 0.6 ml (1.1 equivalents) of 1.06M lithium bis(trimethylsilyl)amide in tetrahydrofuran are added at ambient temperature to 195 mg (0.55 mmol) of methyl 3-methylene-5-(phenylsulfonyl)-2,3,4,5-tetrahydro-1-benzoxepin-7-carboxylate, p...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ccc2c(c1)CCCCO2
c1ccc2c(c1)CCCCO2
c1ccc2c(c1)CCCCO2.c1ccccc1.c1ccccc1
HBr
O1CCCC1.O.ClCCl
null
0.25
BrCc1ccccc1.C=C1COc2ccc(C(=O)OC)cc2C(S(=O)(=O)c2ccccc2)C1>O1CCCC1.O.ClCCl>C=C1COc2ccc(C(=O)OC)cc2C(Cc2ccccc2)(S(=O)(=O)c2ccccc2)C1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ab5491429d1d407e8b0a4e35322d8bac
COC(=O)c1ccc2c(c1)C(Cc1ccccc1)CC(=O)CO2.ClC[P+](c1ccccc1)(c1ccccc1)c1ccccc1>>COC(=O)c1ccc2c(c1)C(Cc1ccccc1)CC(=CCl)CO2
Cl.C(CCC)[Li].[Cl-].ClC[P+](C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1.C(C1=CC=CC=C1)C1CC(COC2=C1C=C(C=C2)C(=O)OC)=O>>C(C1=CC=CC=C1)C1CC(COC2=C1C=C(C=C2)C(=O)OC)=CCl
O=[C:20]1[CH2:19][CH:11]([CH2:12][c:13]2[cH:14][cH:15][cH:16][cH:17][cH:18]2)[c:9]2[c:8]([cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:10]2)[O:24][CH2:23]1.c1ccc([P+](c2ccccc2)(c2ccccc2)[CH2:21][Cl:22])cc1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]2[c:9]([cH:10]1)[CH:11]([CH2:12][c:13]1[cH:14][cH:15][cH:16][cH...
COC(=O)c1ccc2c(c1)C(Cc1ccccc1)CC(=O)CO2.ClC[P+](c1ccccc1)(c1ccccc1)c1ccccc1
COC(=O)c1ccc2c(c1)C(Cc1ccccc1)CC(=CCl)CO2
null
null
ClCCl.O.O1CCCC1
C-C Coupling
Wittig with Phosphonium
33f4b01bff17bc186870f174aa1415cc072a6904bf349e20bef59f70b19d9e13
4ccc953afa1928fe5ef55f22a0c593e017875730e9bc8868efb0bd3550ea5ba6
[CH]=C1COc2ccccc2C(Cc2ccccc2)C1
O=[C;H0;D3;+0:1](-[C:2]-[C:3])-[C:4]-[#8:5]-[c:6].[Cl;D1;H0:7]-[CH2;D2;+0:8]-[P+](-c1:c:c:c:c:c:1)(-c1:c:c:c:c:c:1)-c1:c:c:c:c:c:1>>[C:3]-[C:2]-[C;H0;D3;+0:1](=[CH;D2;+0:8]-[Cl;D1;H0:7])-[C:4]-[#8:5]-[c:6]
53
[{"value": 53.0, "product": "C(C1=CC=CC=C1)C1CC(COC2=C1C=C(C=C2)C(=O)OC)=CCl", "details": "PERCENTYIELD", "is_desired": false}, {"value": 52.5, "product": "C(C1=CC=CC=C1)C1CC(COC2=C1C=C(C=C2)C(=O)OC)=CCl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
1
HOUR
1.1 equivalents of n-butyllithium are added to a suspension of 40 mg (0.12 mmol) of chloromethyltriphenylphosphonium chloride in 3 ml of tetrahydrofuran cooled to 0° C. After stirring for one hour, the ylide is added at 0° C. via a hollow tube to 30 mg (0.1 mmol) of methyl 5-benzyl-3-oxo-2,3,4,5-tetrahydro-1-benzoxepin...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ketone
null
c1ccc2c(c1)CCCCO2.c1ccccc1.c1ccccc1.c1ccccc1
c1ccc2c(c1)CCCCO2
c1ccccc1.c1ccc2c(c1)CCCCO2
HO-
ClCCl.O.O1CCCC1
0
1
COC(=O)c1ccc2c(c1)C(Cc1ccccc1)CC(=O)CO2.ClC[P+](c1ccccc1)(c1ccccc1)c1ccccc1>ClCCl.O.O1CCCC1>COC(=O)c1ccc2c(c1)C(Cc1ccccc1)CC(=CCl)CO2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-fc1f3eb907b64e0188308cae0d70581a
C=C1COc2ccc(C(=O)OC)cc2C(S(=O)(=O)c2ccccc2)C1.C=CCBr>>C=CCC1(S(=O)(=O)c2ccccc2)CC(=C)COc2ccc(C(=O)OC)cc21
C(C=C)Br.Cl.C[Si](C)(C)[N-][Si](C)(C)C.[Li+].C=C1COC2=C(C(C1)S(=O)(=O)C1=CC=CC=C1)C=C(C=C2)C(=O)OC>>C(C=C)C1(CC(COC2=C1C=C(C=C2)C(=O)OC)=C)S(=O)(=O)C2=CC=CC=C2
[CH:4]1([S:5](=[O:6])(=[O:7])[c:8]2[cH:9][cH:10][cH:11][cH:12][cH:13]2)[CH2:14][C:15](=[CH2:16])[CH2:17][O:18][c:19]2[cH:20][cH:21][c:22]([C:23](=[O:24])[O:25][CH3:26])[cH:27][c:28]21.Br[CH2:3][CH:2]=[CH2:1]>>[CH2:1]=[CH:2][CH2:3][C:4]1([S:5](=[O:6])(=[O:7])[c:8]2[cH:9][cH:10][cH:11][cH:12][cH:13]2)[CH2:14][C:15](=[CH2...
C=C1COc2ccc(C(=O)OC)cc2C(S(=O)(=O)c2ccccc2)C1.C=CCBr
C=CCC1(S(=O)(=O)c2ccccc2)CC(=C)COc2ccc(C(=O)OC)cc21
null
null
O1CCCC1.O.ClCCl
C-C Coupling
OtherReaction
79bc13f8b5f05882a3c6a2617dc6381d15033acc40f5dc6619c3addba8aef4fa
4e1ce4e19860a9931e6216ba313479e4494dc60a286d9f70a4527814b3cbb3e2
C=C1COc2ccccc2C(S(=O)(=O)c2ccccc2)C1
Br-[CH2;D2;+0:1]-[C:2]=[C;D1;H2:3].[C;D1;H2:4]=[C:5]1-[C:6]-[CH;D3;+0:7](-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11])-[c:12](:[c:13]):[c:14]-[#8:15]-[C:16]-1>>[C;D1;H2:4]=[C:5]1-[C:6]-[C;H0;D4;+0:7](-[CH2;D2;+0:1]-[C:2]=[C;D1;H2:3])(-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11])-[c:12](:[c:13]):[c:14]-[#8:15]-[C:16]-1
67
[{"value": 67.0, "product": "C(C=C)C1(CC(COC2=C1C=C(C=C2)C(=O)OC)=C)S(=O)(=O)C2=CC=CC=C2", "details": "PERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
0.023 ml (1.1 equivalents) of 1,3-dimethylpropyleneurea and then 0.189 ml (1.1 equivalents) of 1.06M lithium bis(trimethylsilyl)amide in tetrahydrofuran are added at ambient temperature to 61 mg (0.17 mmol) of methyl 3-methylene-5-(phenylsulfonyl)-2,3,4,5-tetrahydro-1-benzoxepin-7-carboxylate, prepared according to exa...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Allyl
Allyl
c1ccc2c(c1)CCCCO2
c1ccc2c(c1)CCCCO2
c1ccccc1.c1ccc2c(c1)CCCCO2
HBr
O1CCCC1.O.ClCCl
null
0.25
C=C1COc2ccc(C(=O)OC)cc2C(S(=O)(=O)c2ccccc2)C1.C=CCBr>O1CCCC1.O.ClCCl>C=CCC1(S(=O)(=O)c2ccccc2)CC(=C)COc2ccc(C(=O)OC)cc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c49d4299a4bd4422926a75399ae58a44
C=C1COc2ccc(C(=O)OC)cc2C(S(=O)(=O)c2ccccc2)C1.CCBr>>C=C1COc2ccc(C(=O)OC)cc2C(CC)(S(=O)(=O)c2ccccc2)C1
C(C)Br.Cl.C[Si](C)(C)[N-][Si](C)(C)C.[Li+].C=C1COC2=C(C(C1)S(=O)(=O)C1=CC=CC=C1)C=C(C=C2)C(=O)OC>>C(C)C1(CC(COC2=C1C=C(C=C2)C(=O)OC)=C)S(=O)(=O)C2=CC=CC=C2
[CH2:1]=[C:2]1[CH2:3][O:4][c:5]2[cH:6][cH:7][c:8]([C:9](=[O:10])[O:11][CH3:12])[cH:13][c:14]2[CH:15]([S:18](=[O:19])(=[O:20])[c:21]2[cH:22][cH:23][cH:24][cH:25][cH:26]2)[CH2:27]1.Br[CH2:16][CH3:17]>>[CH2:1]=[C:2]1[CH2:3][O:4][c:5]2[cH:6][cH:7][c:8]([C:9](=[O:10])[O:11][CH3:12])[cH:13][c:14]2[C:15]([CH2:16][CH3:17])([S:...
C=C1COc2ccc(C(=O)OC)cc2C(S(=O)(=O)c2ccccc2)C1.CCBr
C=C1COc2ccc(C(=O)OC)cc2C(CC)(S(=O)(=O)c2ccccc2)C1
null
null
O1CCCC1.O.ClCCl
C-C Coupling
OtherReaction
0a2d11efff7a4620e79514433af23ac3b11c4e0755c270119fc4a9c5add176d9
f5e5e22797736d188bba28deb76a4cee8e4fee4dca04fe24f733d2ee68a23361
C=C1COc2ccccc2C(S(=O)(=O)c2ccccc2)C1
Br-[CH2;D2;+0:1]-[C;D1;H3:2].[C;D1;H2:3]=[C:4]1-[C:5]-[CH;D3;+0:6](-[#16:7](=[O;D1;H0:8])(=[O;D1;H0:9])-[c:10])-[c:11](:[c:12]):[c:13]-[#8:14]-[C:15]-1>>[C;D1;H2:3]=[C:4]1-[C:5]-[C;H0;D4;+0:6](-[CH2;D2;+0:1]-[C;D1;H3:2])(-[#16:7](=[O;D1;H0:8])(=[O;D1;H0:9])-[c:10])-[c:11](:[c:12]):[c:13]-[#8:14]-[C:15]-1
58
[{"value": 58.0, "product": "C(C)C1(CC(COC2=C1C=C(C=C2)C(=O)OC)=C)S(=O)(=O)C2=CC=CC=C2", "details": "PERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
0.030 ml (1.1 equivalents) of 1,3-dimethylpropyleneurea and then 0.246 ml (1.1 equivalents) of 1.06M lithium bis(trimethylsilyl)amide in tetrahydrofuran are added at ambient temperature to 80 mg (0.22 mmol) of methyl 3-methylene-5-(phenylsulfonyl)-2,3,4,5-tetrahydro-1-benzoxepin-7-carboxylate, prepared according to exa...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ccc2c(c1)CCCCO2
c1ccc2c(c1)CCCCO2
c1ccc2c(c1)CCCCO2.c1ccccc1
HBr
O1CCCC1.O.ClCCl
null
0.25
C=C1COc2ccc(C(=O)OC)cc2C(S(=O)(=O)c2ccccc2)C1.CCBr>O1CCCC1.O.ClCCl>C=C1COc2ccc(C(=O)OC)cc2C(CC)(S(=O)(=O)c2ccccc2)C1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-55d0fc010eec4baeac9b7ff4dcfea9bf
C=C1COc2ccc(C(C)=O)cc2C(S(=O)(=O)c2ccccc2)C1>>C=C1CCc2cc(C(C)O)ccc2OC1
C=C1COC2=C(C(C1)S(=O)(=O)C1=CC=CC=C1)C=C(C=C2)C(C)=O.P(=O)(O)([O-])[O-].[Na+].[Na+].CO.O1CCCC1>>C=C1COC2=C(CC1)C=C(C=C2)C(C)O
O=S(=O)(c1ccccc1)[CH:4]1[CH2:3][C:2](=[CH2:1])[CH2:15][O:14][c:13]2[c:5]1[cH:6][c:7]([C:8]([CH3:9])=[O:10])[cH:11][cH:12]2>>[CH2:1]=[C:2]1[CH2:3][CH2:4][c:5]2[cH:6][c:7]([CH:8]([CH3:9])[OH:10])[cH:11][cH:12][c:13]2[O:14][CH2:15]1
C=C1COc2ccc(C(C)=O)cc2C(S(=O)(=O)c2ccccc2)C1
C=C1CCc2cc(C(C)O)ccc2OC1
null
[Na].[Hg]
O
Reduction
OtherReaction
b53dfd26be6f0f5eafd870670e29785cbeae7e717b7a9db55d5f4c113ab987de
dc5dda88765c78b9cbf727939414381436804136403d7c71b44b3f1693ec9903
C=C1CCc2ccccc2OC1
O=S(=O)(-[CH;D3;+0:1]1-[C:2]-[C:3](=[C;D1;H2:4])-[C:5]-[#8:6]-[c:7]:[c:8]-1:[c:9]:[c:10](-[C;H0;D3;+0:11](-[C;D1;H3:12])=[O;H0;D1;+0:13]):[c:14])-c1:c:c:c:c:c:1>>[C;D1;H2:4]=[C:3]1-[C:5]-[#8:6]-[c:7]:[c:8](:[c:9]:[c:10](-[CH;D3;+0:11](-[C;D1;H3:12])-[OH;D1;+0:13]):[c:14])-[CH2;D2;+0:1]-[C:2]-1
80.7
[{"value": 80.7, "product": "C=C1COC2=C(CC1)C=C(C=C2)C(C)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
3.14 mg (6.82 mmol) of 5% sodium amalgam are added portionwise at 0° C. to 389 mg (1.14 mmol) of 1-[3-methylene-5-(phenylsulfonyl)-2,3,4,5-tetrahydro-1-benzoxepin-7-yl]ethanone, prepared according to example 13, and 648 mg (4.55 mmol) of sodium hydrogenphosphate in suspension in 50 ml of a 1/1 methanol/tetrahydrofuran ...
10.6084/m9.figshare.5104873.v1
null
Ketone.Sulfone
Secondary alcohol
c1ccccc1.c1ccc2c(c1)CCCCO2
c1ccc2c(c1)CCCCO2
c1ccc2c(c1)CCCCO2
HO-
[Na].[Hg].O
null
4
C=C1COc2ccc(C(C)=O)cc2C(S(=O)(=O)c2ccccc2)C1>[Na].[Hg].O>C=C1CCc2cc(C(C)O)ccc2OC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f249fafa738e4090a7c960870da6049d
C=C1CCc2cc(C(C)O)ccc2OC1.O>>CC(=O)c1ccc2c(c1)CCC(=O)CO2
C(Cl)(Cl)(Cl)Cl.C(C)#N.O.C=C1COC2=C(CC1)C=C(C=C2)C(C)O.OC(C)(C)C(C)(C)O.S(=S)(=O)([O-])[O-].[Na+].[Na+].I(=O)(=O)(=O)[O-].[Na+]>>C(C)(=O)C=1C=CC2=C(CCC(CO2)=O)C1
C=[C:12]1[CH2:11][CH2:10][c:8]2[c:7]([cH:6][cH:5][c:4]([CH:2]([CH3:1])[OH:3])[cH:9]2)[O:15][CH2:14]1.[OH2:13]>>[CH3:1][C:2](=[O:3])[c:4]1[cH:5][cH:6][c:7]2[c:8]([cH:9]1)[CH2:10][CH2:11][C:12](=[O:13])[CH2:14][O:15]2
C=C1CCc2cc(C(C)O)ccc2OC1.O
CC(=O)c1ccc2c(c1)CCC(=O)CO2
null
O.O.O.[Ru](Cl)(Cl)Cl
ClCCl
Acylation
OtherReaction
181e308f47a6cb823ec8efc486f7eabe7c93f9ba13abfed4b36c8cd5e336f8fc
32fe5d39ad0dd0a3e3ab68a0d9671c9a9e2e108ed9bea7d5de812b68045bda7b
O=C1CCc2ccccc2OC1
C=[C;H0;D3;+0:1](-[C:2]-[C:3])-[C:4]-[#8:5]-[c:6].[C;D1;H3:7]-[CH;D3;+0:8](-[OH;D1;+0:9])-[c:10](:[c:11]):[c:12].[OH2;D0;+0:13]>>[C;D1;H3:7]-[C;H0;D3;+0:8](=[O;H0;D1;+0:9])-[c:10](:[c:11]):[c:12].[C:3]-[C:2]-[C;H0;D3;+0:1](=[O;H0;D1;+0:13])-[C:4]-[#8:5]-[c:6]
55
[{"value": 55.0, "product": "C(C)(=O)C=1C=CC2=C(CCC(CO2)=O)C1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
24
HOUR
4.7 mg (0.023 mmol) of ruthenium chloride trihydrate are added at 0° C. to 188 mg of 1-(3-methylene-2,3,4,5-tetrahydro-1-benzoxepin-7-yl)ethanol as a mixture with its pinacol dimer, prepared according to example 15, and 1.28 g (5.99 mmol) of sodium periodate in solution in a carbon tetrachloride/acetonitrile/water (2/2...
10.6084/m9.figshare.5104873.v1
null
Secondary alcohol.Vinyl
Ketone.Ketone
c1ccc2c(c1)CCCCO2
c1ccc2c(c1)CCCCO2
c1ccc2c(c1)CCCCO2
Other
O.O.O.[Ru](Cl)(Cl)Cl.ClCCl
null
24
C=C1CCc2cc(C(C)O)ccc2OC1.O>O.O.O.[Ru](Cl)(Cl)Cl.ClCCl>CC(=O)c1ccc2c(c1)CCC(=O)CO2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e746e8ecaa2442ba976ac2c8f3d8b065
BrCc1ccccc1.C=C1COc2ccc(C(C)=O)cc2C(S(=O)(=O)c2ccccc2)C1>>C=C1COc2ccc(C(C)=O)cc2C(Cc2ccccc2)(S(=O)(=O)c2ccccc2)C1
C(C1=CC=CC=C1)Br.Cl.C[Si](C)(C)[N-][Si](C)(C)C.[Li+].C=C1COC2=C(C(C1)S(=O)(=O)C1=CC=CC=C1)C=C(C=C2)C(C)=O>>C(C1=CC=CC=C1)C1(CC(COC2=C1C=C(C=C2)C(C)=O)=C)S(=O)(=O)C2=CC=CC=C2
Br[CH2:15][c:16]1[cH:17][cH:18][cH:19][cH:20][cH:21]1.[CH2:1]=[C:2]1[CH2:3][O:4][c:5]2[cH:6][cH:7][c:8]([C:9]([CH3:10])=[O:11])[cH:12][c:13]2[CH:14]([S:22](=[O:23])(=[O:24])[c:25]2[cH:26][cH:27][cH:28][cH:29][cH:30]2)[CH2:31]1>>[CH2:1]=[C:2]1[CH2:3][O:4][c:5]2[cH:6][cH:7][c:8]([C:9]([CH3:10])=[O:11])[cH:12][c:13]2[C:14...
BrCc1ccccc1.C=C1COc2ccc(C(C)=O)cc2C(S(=O)(=O)c2ccccc2)C1
C=C1COc2ccc(C(C)=O)cc2C(Cc2ccccc2)(S(=O)(=O)c2ccccc2)C1
null
null
O1CCCC1.O.ClCCl
C-C Coupling
OtherReaction
0a2d11efff7a4620e79514433af23ac3b11c4e0755c270119fc4a9c5add176d9
f5e5e22797736d188bba28deb76a4cee8e4fee4dca04fe24f733d2ee68a23361
C=C1COc2ccccc2C(Cc2ccccc2)(S(=O)(=O)c2ccccc2)C1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[C;D1;H2:5]=[C:6]1-[C:7]-[CH;D3;+0:8](-[#16:9](=[O;D1;H0:10])(=[O;D1;H0:11])-[c:12])-[c:13](:[c:14]):[c:15]-[#8:16]-[C:17]-1>>[C;D1;H2:5]=[C:6]1-[C:7]-[C;H0;D4;+0:8](-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4])(-[#16:9](=[O;D1;H0:10])(=[O;D1;H0:11])-[c:12])-[c:13](:[c:14]):[c:15]-[#8:16]-[C:...
97
[{"value": 97.0, "product": "C(C1=CC=CC=C1)C1(CC(COC2=C1C=C(C=C2)C(C)=O)=C)S(=O)(=O)C2=CC=CC=C2", "details": "PERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
0.152 ml (2.2 equivalents) of 1,3-dimethylpropyleneurea and then 1.286 ml (2.2 equivalents) of 1.06M lithium bis(trimethylsilyl)amide in tetrahydrofuran are added at ambient temperature to 200 mg (0.58 mmol) of 1-[3-methylene-5-(phenylsulfonyl)-2,3,4,5-tetrahydro-1-benzoxepin-7-yl]ethanone, prepared according to exampl...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ccc2c(c1)CCCCO2
c1ccc2c(c1)CCCCO2
c1ccc2c(c1)CCCCO2.c1ccccc1.c1ccccc1
HBr
O1CCCC1.O.ClCCl
null
0.25
BrCc1ccccc1.C=C1COc2ccc(C(C)=O)cc2C(S(=O)(=O)c2ccccc2)C1>O1CCCC1.O.ClCCl>C=C1COc2ccc(C(C)=O)cc2C(Cc2ccccc2)(S(=O)(=O)c2ccccc2)C1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-141dcc1cc5a140088ea5e68d2399c500
C=C(CCl)CCl.O=Cc1ccccc1O>>C=C(CCl)COc1ccccc1C=O
[I-].[Na+].C([O-])([O-])=O.[K+].[K+].ClCC(=C)CCl.OC1=C(C=O)C=CC=C1>>ClCC(COC1=C(C=O)C=CC=C1)=C
Cl[CH2:5][C:2](=[CH2:1])[CH2:3][Cl:4].[OH:6][c:7]1[cH:8][cH:9][cH:10][cH:11][c:12]1[CH:13]=[O:14]>>[CH2:1]=[C:2]([CH2:3][Cl:4])[CH2:5][O:6][c:7]1[cH:8][cH:9][cH:10][cH:11][c:12]1[CH:13]=[O:14]
C=C(CCl)CCl.O=Cc1ccccc1O
C=C(CCl)COc1ccccc1C=O
null
null
CC(=O)C
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
7e1040116e3a4cf0e8ec5cc7865388d9cd0efabce6d320a1c25a36e411018d8b
d5f4610d46ccc0478471c5bc0fb862644eaf764bbc5d93badb39d54f6ec8e0a5
c1ccccc1
Cl-[CH2;D2;+0:1]-[C:2](-[C:3])=[C;D1;H2:4].[O;D1;H0:5]=[C:6]-[c:7]:[c:8](-[OH;D1;+0:9]):[c:10]>>[C:3]-[C:2](=[C;D1;H2:4])-[CH2;D2;+0:1]-[O;H0;D2;+0:9]-[c:8](:[c:10]):[c:7]-[C:6]=[O;D1;H0:5]
100.2
[{"value": 70.0, "product": "ClCC(COC1=C(C=O)C=CC=C1)=C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 100.2, "product": "ClCC(COC1=C(C=O)C=CC=C1)=C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
45 g (0.3 mol) of sodium iodide, 16.5 (0.12 mol) of potassium carbonate and 17.36 ml (0.15 mol) of 3-chloro-2-chloromethyl-1-propene are added to 10.4 ml (0.1 mol) of 2-hydroxybenzaldehyde in solution in acetone. The mixture is left at reflux of the solvent for 12 hours and then the solvent is evaporated. The medium is...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic alcohol
Ether
null
null
c1ccccc1
HCl
CC(=O)C
null
null
C=C(CCl)CCl.O=Cc1ccccc1O>CC(=O)C>C=C(CCl)COc1ccccc1C=O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-927e297db59546fc924cca8ee753e324
C=C1C=Cc2ccccc2OC1.CS(N)(=O)=O>>OCC1(O)C=Cc2ccccc2OC1
O.C(C)(C)(C)O.C=C1COC2=C(C=C1)C=CC=C2.CS(=O)(=O)N.S([O-])(O)=O.[Na+]>>OCC1(COC2=C(C=C1)C=CC=C2)O
[CH2:2]=[C:3]1[CH:5]=[CH:6][c:7]2[cH:8][cH:9][cH:10][cH:11][c:12]2[O:13][CH2:14]1.CS(N)(=O)=[O:1]>>[OH:1][CH2:2][C:3]1([OH:4])[CH:5]=[CH:6][c:7]2[cH:8][cH:9][cH:10][cH:11][c:12]2[O:13][CH2:14]1
C=C1C=Cc2ccccc2OC1.CS(N)(=O)=O
OCC1(O)C=Cc2ccccc2OC1
null
[Os](=O)(=O)(=O)=O
null
Heteroatom Alkylation and Arylation
OtherReaction
1dd0175b5e5897c05eeacfea9e93da402a49ee0808c6f9f1e145b9bcb566a8d7
3f275d2f23fbd953aef198569e4b9740a8771e7cfb7bc68348b3c74eeaea8c37
C1=Cc2ccccc2OCC1
C-S(-N)(=O)=[O;H0;D1;+0:1].[CH2;D1;+0:2]=[C;H0;D3;+0:3]1-[C:4]-[#8:5]-[c:6]:[c:7]-[C:8]=[C:9]-1>>[O;D1;H1:10]-[C;H0;D4;+0:3]1(-[CH2;D2;+0:2]-[OH;D1;+0:1])-[C:4]-[#8:5]-[c:6]:[c:7]-[C:8]=[C:9]-1
95
[{"value": 95.0, "product": "OCC1(COC2=C(C=C1)C=CC=C2)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
12
HOUR
160 mg (1 mmol) of 3-methylene-2,3-dihydro-1-benzoxepin, prepared according to example 23, are added to a mixture of 250 mg (1 mmol) of osmium tetroxide and 95 mg (1 mmol) of methanesulfonamide dissolved in 10 ml of a 1/1 water/tert-butanol mixture. After 12 hours at ambient temperature, 1.5 g of sodium bisulfite are i...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Vinyl
Primary alcohol.Tertiary alcohol
C1=Cc2ccccc2OCC1
C1=Cc2ccccc2OCC1
C1=Cc2ccccc2OCC1
HO-
[Os](=O)(=O)(=O)=O
null
12
C=C1C=Cc2ccccc2OC1.CS(N)(=O)=O>[Os](=O)(=O)(=O)=O>OCC1(O)C=Cc2ccccc2OC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4aac08ded32d4d21886abfba29f677cd
OCC1(O)C=Cc2ccccc2OC1>>O=C1C=Cc2ccccc2OC1
I(=O)(=O)(=O)[O-].[Na+].OCC1(COC2=C(C=C1)C=CC=C2)O>>O1CC(C=CC2=C1C=CC=C2)=O
OC[C:2]1([OH:1])[CH:3]=[CH:4][c:5]2[cH:6][cH:7][cH:8][cH:9][c:10]2[O:11][CH2:12]1>>[O:1]=[C:2]1[CH:3]=[CH:4][c:5]2[cH:6][cH:7][cH:8][cH:9][c:10]2[O:11][CH2:12]1
OCC1(O)C=Cc2ccccc2OC1
O=C1C=Cc2ccccc2OC1
null
null
O1CCOCC1.O
Miscellaneous
OtherReaction
4c323face09bd7ca7c812bd2d273a27bf3fc8629abb540a58cadbb80a381e3cc
d8333db1a8553533b9f31a51fd46ac10421b6606be90ce648ca3b16dc0428896
O=C1C=Cc2ccccc2OC1
O-C-[C;H0;D4;+0:1]1(-[OH;D1;+0:2])-[C:3]-[#8:4]-[c:5]:[c:6]-[C:7]=[C:8]-1>>[O;H0;D1;+0:2]=[C;H0;D3;+0:1]1-[C:3]-[#8:4]-[c:5]:[c:6]-[C:7]=[C:8]-1
70
[{"value": 70.0, "product": "O1CC(C=CC2=C1C=CC=C2)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 69.2, "product": "O1CC(C=CC2=C1C=CC=C2)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
4×28.5 mg (0.55 mmol) of sodium periodate are added in four equal portions over 30 minutes to 106 mg (0.55 mmol) of 3-(hydroxymethyl)-2,3-dihydro-1-benzoxepin-3-ol, prepared according to example 24, in solution in 3 ml of a 3/7 dioxane/water mixture. After stirring at ambient temperature for 2 hours, the medium is filt...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Tertiary alcohol
Ketone
C1=Cc2ccccc2OCC1
C1=Cc2ccccc2OCC1
C1=Cc2ccccc2OCC1
HO-
O1CCOCC1.O
null
2
OCC1(O)C=Cc2ccccc2OC1>O1CCOCC1.O>O=C1C=Cc2ccccc2OC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-acfe2cd6cd61488092e8115fdd52e651
ClC[P+](c1ccccc1)(c1ccccc1)c1ccccc1.O=C1C=Cc2ccccc2OC1>>ClC=C1C=Cc2ccccc2OC1
C(CCC)[Li].[Cl-].ClC[P+](C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1.O1CC(C=CC2=C1C=CC=C2)=O>>ClC=C1COC2=C(C=C1)C=CC=C2
c1ccc([P+](c2ccccc2)(c2ccccc2)[CH2:2][Cl:1])cc1.O=[C:3]1[CH:4]=[CH:5][c:6]2[cH:7][cH:8][cH:9][cH:10][c:11]2[O:12][CH2:13]1>>[Cl:1][CH:2]=[C:3]1[CH:4]=[CH:5][c:6]2[cH:7][cH:8][cH:9][cH:10][c:11]2[O:12][CH2:13]1
ClC[P+](c1ccccc1)(c1ccccc1)c1ccccc1.O=C1C=Cc2ccccc2OC1
ClC=C1C=Cc2ccccc2OC1
null
null
O1CCCC1.CCCCC
C-C Coupling
Wittig with Phosphonium
539d98d0a68c79c0ce64fb9b77faf88c2e8998170a817390f2eb321da849bd7d
4ccc953afa1928fe5ef55f22a0c593e017875730e9bc8868efb0bd3550ea5ba6
[CH]=C1C=Cc2ccccc2OC1
O=[C;H0;D3;+0:1]1-[C:2]-[#8:3]-[c:4]:[c:5]-[C:6]=[C:7]-1.[Cl;D1;H0:8]-[CH2;D2;+0:9]-[P+](-c1:c:c:c:c:c:1)(-c1:c:c:c:c:c:1)-c1:c:c:c:c:c:1>>[Cl;D1;H0:8]-[CH;D2;+0:9]=[C;H0;D3;+0:1]1-[C:2]-[#8:3]-[c:4]:[c:5]-[C:6]=[C:7]-1
52
[{"value": 52.0, "product": "ClC=C1COC2=C(C=C1)C=CC=C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 51.9, "product": "ClC=C1COC2=C(C=C1)C=CC=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
1
HOUR
1.1 eq. of n-butyllithium are added to 104 mg (0.3 mmol) of chloromethyltriphenylphosphonium chloride in solution in tetrahydrofuran cooled to 0° C. After stirring for one hour, 40 mg (0.25 mmol) of 1-benzoxepin-3(2H)-one, prepared according to example 25, are added at ambient temperature and the mixture is left for 1 ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ketone
null
c1ccccc1.c1ccccc1.c1ccccc1.C1=Cc2ccccc2OCC1
C1=Cc2ccccc2OCC1
C1=Cc2ccccc2OCC1
HO-
O1CCCC1.CCCCC
0
1
ClC[P+](c1ccccc1)(c1ccccc1)c1ccccc1.O=C1C=Cc2ccccc2OC1>O1CCCC1.CCCCC>ClC=C1C=Cc2ccccc2OC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4b1e0f16b5354988b0a789b4e223685d
CC(=O)c1ccc2c(c1)C(S(=O)(=O)c1ccccc1)CC(=O)CO2>>CC(=O)c1ccc2c(c1)C=CC(=O)CO2
N12CCCCCC2=NCCC1.C(C)(=O)C=1C=CC2=C(C(CC(CO2)=O)S(=O)(=O)C2=CC=CC=C2)C1.O.Cl>>C(C)(=O)C=1C=CC2=C(C=CC(CO2)=O)C1
O=S(=O)(c1ccccc1)[CH:10]1[c:8]2[c:7]([cH:6][cH:5][c:4]([C:2]([CH3:1])=[O:3])[cH:9]2)[O:15][CH2:14][C:12](=[O:13])[CH2:11]1>>[CH3:1][C:2](=[O:3])[c:4]1[cH:5][cH:6][c:7]2[c:8]([cH:9]1)[CH:10]=[CH:11][C:12](=[O:13])[CH2:14][O:15]2
CC(=O)c1ccc2c(c1)C(S(=O)(=O)c1ccccc1)CC(=O)CO2
CC(=O)c1ccc2c(c1)C=CC(=O)CO2
null
null
ClCCl
Functional Group Interconversion
Cleavage of sulfons and sulfoxides
0f56729427ccdf9758e239f6d9c2624c4c21e1338166c34e8aac92b936db11eb
048fee841aa83d6ccd159043413f753eba30ed171e5ec6a25efdb332fddc5ab3
O=C1C=Cc2ccccc2OC1
O=S(=O)(-[CH;D3;+0:1]1-[CH2;D2;+0:2]-[C:3](=[O;D1;H0:4])-[C:5]-[#8:6]-[c:7]:[c:8]-1:[c:9])-c1:c:c:c:c:c:1>>[O;D1;H0:4]=[C:3]1-[C:5]-[#8:6]-[c:7]:[c:8](:[c:9])-[CH;D2;+0:1]=[CH;D2;+0:2]-1
null
[]
null
null
null
null
0.084 ml (1.05 equivalents) of 1,8-diazabicyclo[5.4.0]undec-7-ene is added at ambient temperature, under nitrogen, to 184 mg (0.53 mmol) of 7-acetyl-5-(phenylsulfonyl)-4,5-dihydro-1-benzoxepin-3(2H)-one, prepared according to example 14, in suspension in 20 ml of dichloromethane. From the addition of the base, the medi...
10.6084/m9.figshare.5104873.v1
null
Ketone.Sulfone
Ketone
c1ccccc1.c1ccc2c(c1)CCCCO2
C1=Cc2ccccc2OCC1
C1=Cc2ccccc2OCC1
HO-
ClCCl
null
null
CC(=O)c1ccc2c(c1)C(S(=O)(=O)c1ccccc1)CC(=O)CO2>ClCCl>CC(=O)c1ccc2c(c1)C=CC(=O)CO2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-eb8285bcd2b84ff3b1be95b859facf7a
COC(=O)c1ccc2c(c1)C(S(=O)(=O)c1ccccc1)CC(=O)CO2>>COC(=O)c1ccc2c(c1)C=CC(=O)CO2
N12CCCCCC2=NCCC1.O=C1COC2=C(C(C1)S(=O)(=O)C1=CC=CC=C1)C=C(C=C2)C(=O)OC.O.Cl>>O=C1COC2=C(C=C1)C=C(C=C2)C(=O)OC
O=S(=O)(c1ccccc1)[CH:11]1[c:9]2[c:8]([cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:10]2)[O:16][CH2:15][C:13](=[O:14])[CH2:12]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]2[c:9]([cH:10]1)[CH:11]=[CH:12][C:13](=[O:14])[CH2:15][O:16]2
COC(=O)c1ccc2c(c1)C(S(=O)(=O)c1ccccc1)CC(=O)CO2
COC(=O)c1ccc2c(c1)C=CC(=O)CO2
null
null
ClCCl
Functional Group Interconversion
Cleavage of sulfons and sulfoxides
0f56729427ccdf9758e239f6d9c2624c4c21e1338166c34e8aac92b936db11eb
048fee841aa83d6ccd159043413f753eba30ed171e5ec6a25efdb332fddc5ab3
O=C1C=Cc2ccccc2OC1
O=S(=O)(-[CH;D3;+0:1]1-[CH2;D2;+0:2]-[C:3](=[O;D1;H0:4])-[C:5]-[#8:6]-[c:7]:[c:8]-1:[c:9])-c1:c:c:c:c:c:1>>[O;D1;H0:4]=[C:3]1-[C:5]-[#8:6]-[c:7]:[c:8](:[c:9])-[CH;D2;+0:1]=[CH;D2;+0:2]-1
null
[]
null
null
null
null
0.084 ml (1.05 equivalents) of 1,8-diazabicyclo[5.4.0]undec-7-ene is added at ambient temperature to 217 mg (0.6 mmol) of methyl 3-oxo-5-(phenylsulfonyl)-2,3,4,5-tetrahydro-1-benzoxepin-7-carboxylate, prepared according to example 2, in suspension in 20 ml of dichloromethane. From the addition of the base, the medium b...
10.6084/m9.figshare.5104873.v1
null
Ketone.Sulfone
Ketone
c1ccccc1.c1ccc2c(c1)CCCCO2
C1=Cc2ccccc2OCC1
C1=Cc2ccccc2OCC1
HO-
ClCCl
null
null
COC(=O)c1ccc2c(c1)C(S(=O)(=O)c1ccccc1)CC(=O)CO2>ClCCl>COC(=O)c1ccc2c(c1)C=CC(=O)CO2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-7b9fffa4797c49fc8b9d7d7c2063b12c
COC(=O)c1ccc2c(c1)C=CC(=O)CO2.ClC[P+](c1ccccc1)(c1ccccc1)c1ccccc1>>COC(=O)c1ccc2c(c1)C=CC(=CCl)CO2
Cl.C(CCC)[Li].[Cl-].ClC[P+](C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1.O=C1COC2=C(C=C1)C=C(C=C2)C(=O)OC>>ClC=C1COC2=C(C=C1)C=C(C=C2)C(=O)OC
O=[C:13]1[CH:12]=[CH:11][c:9]2[c:8]([cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:10]2)[O:17][CH2:16]1.c1ccc([P+](c2ccccc2)(c2ccccc2)[CH2:14][Cl:15])cc1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]2[c:9]([cH:10]1)[CH:11]=[CH:12][C:13](=[CH:14][Cl:15])[CH2:16][O:17]2
COC(=O)c1ccc2c(c1)C=CC(=O)CO2.ClC[P+](c1ccccc1)(c1ccccc1)c1ccccc1
COC(=O)c1ccc2c(c1)C=CC(=CCl)CO2
null
null
ClCCl.O.O1CCCC1
C-C Coupling
Wittig with Phosphonium
539d98d0a68c79c0ce64fb9b77faf88c2e8998170a817390f2eb321da849bd7d
4ccc953afa1928fe5ef55f22a0c593e017875730e9bc8868efb0bd3550ea5ba6
[CH]=C1C=Cc2ccccc2OC1
O=[C;H0;D3;+0:1]1-[C:2]=[C:3]-[c:4]:[c:5]-[#8:6]-[C:7]-1.[Cl;D1;H0:8]-[CH2;D2;+0:9]-[P+](-c1:c:c:c:c:c:1)(-c1:c:c:c:c:c:1)-c1:c:c:c:c:c:1>>[Cl;D1;H0:8]-[CH;D2;+0:9]=[C;H0;D3;+0:1]1-[C:2]=[C:3]-[c:4]:[c:5]-[#8:6]-[C:7]-1
97.3
[{"value": 96.0, "product": "ClC=C1COC2=C(C=C1)C=C(C=C2)C(=O)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 97.3, "product": "ClC=C1COC2=C(C=C1)C=C(C=C2)C(=O)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
1
HOUR
1.3 equivalents of n-butyllithium are added to a suspension of 122 mg (0.35 mmol) of chloromethyltriphenylphosphonium chloride in tetrahydrofuran cooled to 0° C. After stirring for one hour, the ylide is added at 0° C., via a hollow tube, to 55 mg (0.25 mmol) of methyl 3-oxo-2,3-dihydro-1-benzoxepin-7-carboxylate, prep...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ketone
null
C1=Cc2ccccc2OCC1.c1ccccc1.c1ccccc1.c1ccccc1
C1=Cc2ccccc2OCC1
C1=Cc2ccccc2OCC1
HO-
ClCCl.O.O1CCCC1
0
1
COC(=O)c1ccc2c(c1)C=CC(=O)CO2.ClC[P+](c1ccccc1)(c1ccccc1)c1ccccc1>ClCCl.O.O1CCCC1>COC(=O)c1ccc2c(c1)C=CC(=CCl)CO2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-da6893c26e3d4b92944c5b272507bc23
COC(=O)C1(O)C=CC=CC1.O=C(O)C(F)(F)F>>COC(=O)c1ccc(O)c(C=O)c1
O.FC(C(=O)O)(F)F.OC1(C(=O)OC)CC=CC=C1.C1N2CN3CN1CN(C2)C3>>C(=O)C=1C=C(C(=O)OC)C=CC1O
[CH3:1][O:2][C:3](=[O:4])[C:5]1([OH:9])[CH:6]=[CH:7][CH:8]=[CH:10][CH2:13]1.O[C:11](C(F)(F)F)=[O:12]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([OH:9])[c:10]([CH:11]=[O:12])[cH:13]1
COC(=O)C1(O)C=CC=CC1.O=C(O)C(F)(F)F
COC(=O)c1ccc(O)c(C=O)c1
null
null
null
Aromatic Heterocycle Formation
OtherReaction
5da8c048780f74aedff48c41c78ed48a1f83f77fbd8859abf216996356091e23
74cae3b1f515707702b22095223480fe6c095d2957b7b866e70054945e4d6312
c1ccccc1
F-C(-F)(-F)-[C;H0;D3;+0:1](-O)=[O;D1;H0:2].[C;D1;H3:3]-[#8:4]-[C:5](=[O;D1;H0:6])-[C;H0;D4;+0:7]1(-[OH;D1;+0:8])-[CH2;D2;+0:9]-[CH;D2;+0:10]=[CH;D2;+0:11]-[CH;D2;+0:12]=[CH;D2;+0:13]-1>>[C;D1;H3:3]-[#8:4]-[C:5](=[O;D1;H0:6])-[c;H0;D3;+0:7]1:[cH;D2;+0:9]:[c;H0;D3;+0:10](-[CH;D2;+0:1]=[O;D1;H0:2]):[c;H0;D3;+0:11](-[OH;D1...
37
[{"value": 37.0, "product": "C(=O)C=1C=C(C(=O)OC)C=CC1O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
24 ml of trifluoroacetic acid are added at 0° C. to a mixture of 4.56 g (30 mmol) of methyl 1-hydroxybenzoate and 8.64 g (60 mmol) of hexamethylenetetramine. The solution is brought to reflux and is stirred for 2 hours. After cooling, the solution is diluted with water to 50 ml. The solution is stirred overnight at amb...
10.6084/m9.figshare.5104873.v1
null
Trifluoro group.Carboxylic acid.Ester.Tertiary alcohol.Conjugated diene
Aldehyde.Ester.Aromatic alcohol
C1=CCCC=C1
c1ccccc1
c1ccccc1
HF
null
null
2
COC(=O)C1(O)C=CC=CC1.O=C(O)C(F)(F)F>>COC(=O)c1ccc(O)c(C=O)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0276606162d6416e9332d1d0a1662348
C=C(CCl)CCl.COC(=O)c1ccc(O)c(C=O)c1>>C=C(CCl)COc1ccc(C(=O)OC)cc1C=O
Cl.CN(C=O)C.ClCC(=C)CCl.C(=O)C=1C=C(C(=O)OC)C=CC1O>>ClCC(COC1=C(C=C(C(=O)OC)C=C1)C=O)=C
Cl[CH2:5][C:2](=[CH2:1])[CH2:3][Cl:4].[OH:6][c:7]1[cH:8][cH:9][c:10]([C:11](=[O:12])[O:13][CH3:14])[cH:15][c:16]1[CH:17]=[O:18]>>[CH2:1]=[C:2]([CH2:3][Cl:4])[CH2:5][O:6][c:7]1[cH:8][cH:9][c:10]([C:11](=[O:12])[O:13][CH3:14])[cH:15][c:16]1[CH:17]=[O:18]
C=C(CCl)CCl.COC(=O)c1ccc(O)c(C=O)c1
C=C(CCl)COc1ccc(C(=O)OC)cc1C=O
null
[I-].C(CCC)[N+](CCCC)(CCCC)CCCC
O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
7e1040116e3a4cf0e8ec5cc7865388d9cd0efabce6d320a1c25a36e411018d8b
d5f4610d46ccc0478471c5bc0fb862644eaf764bbc5d93badb39d54f6ec8e0a5
c1ccccc1
Cl-[CH2;D2;+0:1]-[C:2](-[C:3])=[C;D1;H2:4].[O;D1;H0:5]=[C:6]-[c:7]:[c:8](-[OH;D1;+0:9]):[c:10]>>[C:3]-[C:2](=[C;D1;H2:4])-[CH2;D2;+0:1]-[O;H0;D2;+0:9]-[c:8](:[c:10]):[c:7]-[C:6]=[O;D1;H0:5]
52.4
[{"value": 52.0, "product": "ClCC(COC1=C(C=C(C(=O)OC)C=C1)C=O)=C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 52.4, "product": "ClCC(COC1=C(C=C(C(=O)OC)C=C1)C=O)=C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
26
HOUR
45 ml of dimethylformamide and then 1.15 ml (9.95 mmol) of 2-chloromethyl-3-chloro-1-propene are added under argon to 717 mg (3.98 mmol) of methyl 3-formyl-4-hydroxybenzoate as a mixture with 1.055 g (9.95 mmol) and 440 mg (1.195 mmol) of tetrabutylammonium iodide. The solution is stirred for 26 hours and then water is...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic alcohol
Ether
null
null
c1ccccc1
HCl
[I-].C(CCC)[N+](CCCC)(CCCC)CCCC.O
null
26
C=C(CCl)CCl.COC(=O)c1ccc(O)c(C=O)c1>[I-].C(CCC)[N+](CCCC)(CCCC)CCCC.O>C=C(CCl)COc1ccc(C(=O)OC)cc1C=O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4013f461401d4a6c8b6775ee63a3fbac
C=C(CCl)COc1ccc(C(=O)OC)cc1C=O.[I-]>>C=C(CI)COc1ccc(C(=O)OC)cc1C=O
[I-].[Na+].ClCC(COC1=C(C=C(C(=O)OC)C=C1)C=O)=C>>ICC(COC1=C(C=C(C(=O)OC)C=C1)C=O)=C
Cl[CH2:3][C:2](=[CH2:1])[CH2:5][O:6][c:7]1[cH:8][cH:9][c:10]([C:11](=[O:12])[O:13][CH3:14])[cH:15][c:16]1[CH:17]=[O:18].[I-:4]>>[CH2:1]=[C:2]([CH2:3][I:4])[CH2:5][O:6][c:7]1[cH:8][cH:9][c:10]([C:11](=[O:12])[O:13][CH3:14])[cH:15][c:16]1[CH:17]=[O:18]
C=C(CCl)COc1ccc(C(=O)OC)cc1C=O.[I-]
C=C(CI)COc1ccc(C(=O)OC)cc1C=O
null
null
CC(=O)C
Functional Group Interconversion
OtherReaction
e944a2acb95a43a23818321f2ac2f96ba2f2b8d34f52c1cfd1e3802d2403177f
e2ca6f9fe1078a3836d617896a4e5cc310fb155ca459b021e2b549b3e61f1df7
c1ccccc1
Cl-[CH2;D2;+0:1]-[C:2](-[C:3])=[C;D1;H2:4].[I-;H0;D0:5]>>[C:3]-[C:2](=[C;D1;H2:4])-[CH2;D2;+0:1]-[I;H0;D1;+0:5]
91
[{"value": 91.0, "product": "ICC(COC1=C(C=C(C(=O)OC)C=C1)C=O)=C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 90.8, "product": "ICC(COC1=C(C=C(C(=O)OC)C=C1)C=O)=C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
5
HOUR
375 mg (2.5 mmol) of sodium iodide are added to 560 mg (2.08 mmol) of methyl 4-{[2-(chloromethyl)-2-propenyl]oxy}-3-formylbenzoate in solution in 20 ml of acetone. The solution is brought to reflux and is stirred for 5 hours with the exclusion of light. After the usual treatments, 680 mg (91%) of methyl 4-{[2-(iodometh...
10.6084/m9.figshare.5104873.v1
null
Primary halide
Primary halide
null
null
c1ccccc1
Other
CC(=O)C
null
5
C=C(CCl)COc1ccc(C(=O)OC)cc1C=O.[I-]>CC(=O)C>C=C(CI)COc1ccc(C(=O)OC)cc1C=O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f5df823ed3eb434a8e25c7760acc0ac2
C=C(CCl)COc1ccc(C(=O)OC)cc1C=O>>C=C1C=Cc2cc(C(=O)OC)ccc2OC1
ClCC(COC1=C(C=C(C(=O)OC)C=C1)C=O)=C.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.ICC(COC1=C(C=C(C(=O)OC)C=C1)C=O)=C.C[O-].[Na+]>>C=C1COC2=C(C=C1)C=C(C=C2)C(=O)OC
O=[CH:4][c:5]1[cH:6][c:7]([C:8](=[O:9])[O:10][CH3:11])[cH:12][cH:13][c:14]1[O:15][CH2:16][C:2](=[CH2:1])[CH2:3]Cl>>[CH2:1]=[C:2]1[CH:3]=[CH:4][c:5]2[cH:6][c:7]([C:8](=[O:9])[O:10][CH3:11])[cH:12][cH:13][c:14]2[O:15][CH2:16]1
C=C(CCl)COc1ccc(C(=O)OC)cc1C=O
C=C1C=Cc2cc(C(=O)OC)ccc2OC1
null
null
C(C)#N.CO
C-C Coupling
OtherReaction
cd8aa2006e08ebd6c5752a804163d33604e551cb274de5cfef9b1f643743b122
a3dca447376ff0c6fe3968bb1ab0785c8926c417c53ba2b61f8ebdb52a7e5a2a
C=C1C=Cc2ccccc2OC1
Cl-[CH2;D2;+0:1]-[C:2](-[C:3])=[C;D1;H2:4].O=[CH;D2;+0:5]-[c:6](:[c:7]):[c:8]>>[C:3]-[C:2](=[C;D1;H2:4])-[CH;D2;+0:1]=[CH;D2;+0:5]-[c:6](:[c:7]):[c:8]
54
[{"value": 54.0, "product": "C=C1COC2=C(C=C1)C=C(C=C2)C(=O)OC", "details": "PERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
333 mg (1 mmol) of a 60/40 mixture of methyl 4-{[2-(iodomethyl)-2-propenyl]oxy}-3-formylbenzoate and of methyl 4-{[2-(chloromethyl)-2-propenyl]oxy}-3-formylbenzoate and then 297 mg (1.133 mmol) of triphenylphosphine are successively introduced into the 50 ml single-necked flask. The combined mixture is subjected to a s...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aldehyde
null
null
C1=Cc2ccccc2OCC1
C1=Cc2ccccc2OCC1
HCl
C(C)#N.CO
null
1
C=C(CCl)COc1ccc(C(=O)OC)cc1C=O>C(C)#N.CO>C=C1C=Cc2cc(C(=O)OC)ccc2OC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4ac67eff34a54ca7bf3f8d6b1731f03d
C=C1C=Cc2cc(C(=O)OC)ccc2OC1>>C=C1C=Cc2cc(C(=O)O)ccc2OC1
[OH-].[K+].C=C1COC2=C(C=C1)C=C(C=C2)C(=O)OC.Cl>>C=C1COC2=C(C=C1)C=C(C=C2)C(=O)O
C[O:10][C:8]([c:7]1[cH:6][c:5]2[c:13]([cH:12][cH:11]1)[O:14][CH2:15][C:2](=[CH2:1])[CH:3]=[CH:4]2)=[O:9]>>[CH2:1]=[C:2]1[CH:3]=[CH:4][c:5]2[cH:6][c:7]([C:8](=[O:9])[OH:10])[cH:11][cH:12][c:13]2[O:14][CH2:15]1
C=C1C=Cc2cc(C(=O)OC)ccc2OC1
C=C1C=Cc2cc(C(=O)O)ccc2OC1
null
null
C(C)O
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
C=C1C=Cc2ccccc2OC1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]
88.2
[{"value": 88.0, "product": "C=C1COC2=C(C=C1)C=C(C=C2)C(=O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 88.2, "product": "C=C1COC2=C(C=C1)C=C(C=C2)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
1.2 g of potassium hydroxide pellets are added to 4 g (18.5 mmol) of methyl 3-methylene-2,3-dihydro-1-benzoxepin-7-carboxylate, prepared according to example 35, in solution in 20 ml of 80% aqueous ethanol. The medium is brought to reflux for 4 hours and then, after cooling, is treated with 1N hydrochloric acid until p...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
C1=Cc2ccccc2OCC1
Other
C(C)O
null
null
C=C1C=Cc2cc(C(=O)OC)ccc2OC1>C(C)O>C=C1C=Cc2cc(C(=O)O)ccc2OC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d7c1f62e8e2547cea838bf05bb3c09f8
C=C1C=Cc2cc(C(=O)O)ccc2OC1.Nc1ccccc1>>C=C1C=Cc2cc(C(=O)Nc3ccccc3)ccc2OC1
[Cl-].COC1=NC(=NC(=N1)OC)[N+]1(CCOCC1)C.NC1=CC=CC=C1.C=C1COC2=C(C=C1)C=C(C=C2)C(=O)O>>C=C1COC2=C(C=C1)C=C(C=C2)C(=O)NC2=CC=CC=C2
O[C:8]([c:7]1[cH:6][c:5]2[c:19]([cH:18][cH:17]1)[O:20][CH2:21][C:2](=[CH2:1])[CH:3]=[CH:4]2)=[O:9].[NH2:10][c:11]1[cH:12][cH:13][cH:14][cH:15][cH:16]1>>[CH2:1]=[C:2]1[CH:3]=[CH:4][c:5]2[cH:6][c:7]([C:8](=[O:9])[NH:10][c:11]3[cH:12][cH:13][cH:14][cH:15][cH:16]3)[cH:17][cH:18][c:19]2[O:20][CH2:21]1
C=C1C=Cc2cc(C(=O)O)ccc2OC1.Nc1ccccc1
C=C1C=Cc2cc(C(=O)Nc3ccccc3)ccc2OC1
null
null
CO
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
C=C1C=Cc2cc(C(=O)Nc3ccccc3)ccc2OC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9])-[c:3](:[c:4]):[c:5]
49
[{"value": 49.0, "product": "C=C1COC2=C(C=C1)C=C(C=C2)C(=O)NC2=CC=CC=C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 18.0, "product": "C=C1COC2=C(C=C1)C=C(C=C2)C(=O)NC2=CC=CC=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
24
HOUR
1.12 g (4.07 mmol) of 4-(4,6-dimethoxy-1,3,5-triazin-2-yl)-4-methylmorpholinium chloride and then 0.379 g (4.07 mmol) of aniline are successively added to 0.75 g (3.7 mmol) of 3-methylene-2,3-dihydro-1-benzoxepin-7-carboxylic acid, prepared according to example 40, in solution in 25 ml of methanol. The medium is stirre...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
C1=Cc2ccccc2OCC1.c1ccccc1
HO-
CO
null
24
C=C1C=Cc2cc(C(=O)O)ccc2OC1.Nc1ccccc1>CO>C=C1C=Cc2cc(C(=O)Nc3ccccc3)ccc2OC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-2bc99a6f11a2488abd035af078d29166
C=C1C=Cc2cc(C(=O)OC)ccc2OC1.CC[C@@H]1CN2CC[C@@H]1C[C@@H]2[C@H](Oc1nnc(O[C@H](c2ccnc3ccc(OC)cc23)[C@H]2C[C@@H]3CCN2C[C@@H]3CC)c2ccccc12)c1ccnc2ccc(OC)cc12.CS(N)(=O)=O>>COC(=O)c1ccc2c(c1)C=CC(O)(CO)CO2
S(=O)([O-])OS(=O)[O-].[Na+].[Na+].C(C)(C)(C)O.O.CC[C@@H]1CN2CC[C@@H]1C[C@@H]2[C@@H](C3=C4C=C(C=CC4=NC=C3)OC)OC5=NN=C(C6=CC=CC=C65)O[C@@H]([C@H]7C[C@@H]8CCN7C[C@@H]8CC)C9=C1C=C(C=CC1=NC=C9)OC.CS(=O)(=O)N.C(C)(C)(C)O.O.C=C1COC2=C(C=C1)C=C(C=C2)C(=O)OC>>OC1(COC2=C(C=C1)C=C(C=C2)C(=O)OC)CO
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]2[c:9]([cH:10]1)[CH:11]=[CH:12][C:13](=[CH2:15])[CH2:17][O:18]2.CC[C@@H]1CN2CC[C@@H]1C[C@@H]2[C@@H](c1ccnc2ccc(OC)cc12)[O:14]c1nnc(O[C@H](c2ccnc3ccc(OC)cc23)[C@H]2C[C@@H]3CCN2C[C@@H]3CC)c2ccccc12.CS(N)(=O)=[O:16]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]2[c:9]([cH...
C=C1C=Cc2cc(C(=O)OC)ccc2OC1.CC[C@@H]1CN2CC[C@@H]1C[C@@H]2[C@H](Oc1nnc(O[C@H](c2ccnc3ccc(OC)cc23)[C@H]2C[C@@H]3CCN2C[C@@H]3CC)c2ccccc12)c1ccnc2ccc(OC)cc12.CS(N)(=O)=O
COC(=O)c1ccc2c(c1)C=CC(O)(CO)CO2
null
null
ClCCl
Heteroatom Alkylation and Arylation
OtherReaction
6e442f716680a56517ea1ae63548e6febe18422775fb7d10a8f7f59df9256545
f275e2b911856e91a6e8071aae74404b344120b5a7e2bb0af9b98d866ffebd4b
C1=Cc2ccccc2OCC1
C-C-[C@H]1-C-N2-C-C-[C@H]-1-C-[C@@H]-2-[C@H](-O-c1:n:n:c(-[O;H0;D2;+0:1]-[C@@H](-[C@H]2-C-[C@H]3-C-C-N-2-C-[C@H]-3-C-C)-c2:c:c:n:c3:c:c:c(-O-C):c:c:2:3):c2:c:c:c:c:c:1:2)-c1:c:c:n:c2:c:c:c(-O-C):c:c:1:2.C-S(-N)(=O)=[O;H0;D1;+0:2].[CH2;D1;+0:3]=[C;H0;D3;+0:4]1-[C:5]=[C:6]-[c:7]:[c:8]-[#8:9]-[C:10]-1>>[OH;D1;+0:1]-[C;H0;...
100
[{"value": 100.0, "product": "OC1(COC2=C(C=C1)C=C(C=C2)C(=O)OC)CO", "details": "PERCENTYIELD", "is_desired": false}]
null
null
4
DAY
21 g (7 equivalents) of AD-mix-α and 1.31 g (13.8 mmol) of methanesulfonamide dissolved in 75 ml of a 1/1 tert-butyl alcohol/water mixture are added at ambient temperature to 3 g (13.8 mmol) of methyl 3-methylene-2,3-dihydro-1-benzoxepin-7-carboxylate, prepared according to example 35, in suspension in 20 ml of a 1/1 t...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Ether.Ether.Ether.Ether.Tertiary amine.Tertiary amine.Vinyl
Primary alcohol.Tertiary alcohol
C1=Cc2ccccc2OCC1.c1ccc2ncccc2c1.c1ccc2ncccc2c1.c1ccc2cnncc2c1.C1CN2CCC1CC2.C1CN2CCC1CC2
C1=Cc2ccccc2OCC1
C1=Cc2ccccc2OCC1
HO-
ClCCl
null
96
C=C1C=Cc2cc(C(=O)OC)ccc2OC1.CC[C@@H]1CN2CC[C@@H]1C[C@@H]2[C@H](Oc1nnc(O[C@H](c2ccnc3ccc(OC)cc23)[C@H]2C[C@@H]3CCN2C[C@@H]3CC)c2ccccc12)c1ccnc2ccc(OC)cc12.CS(N)(=O)=O>ClCCl>COC(=O)c1ccc2c(c1)C=CC(O)(CO)CO2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a795c22745ff44ec960187343b96c62e
COC(=O)c1ccc2c(c1)C=CC(O)(CO)CO2>>COC(=O)c1ccc2c(c1)C=CC(=O)CO2
I(=O)(=O)(=O)[O-].[Na+].OC1(COC2=C(C=C1)C=C(C=C2)C(=O)OC)CO>>O=C1COC2=C(C=C1)C=C(C=C2)C(=O)OC
OC[C:13]1([OH:14])[CH:12]=[CH:11][c:9]2[c:8]([cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:10]2)[O:16][CH2:15]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]2[c:9]([cH:10]1)[CH:11]=[CH:12][C:13](=[O:14])[CH2:15][O:16]2
COC(=O)c1ccc2c(c1)C=CC(O)(CO)CO2
COC(=O)c1ccc2c(c1)C=CC(=O)CO2
null
null
O1CCOCC1.O
Miscellaneous
OtherReaction
4c323face09bd7ca7c812bd2d273a27bf3fc8629abb540a58cadbb80a381e3cc
d8333db1a8553533b9f31a51fd46ac10421b6606be90ce648ca3b16dc0428896
O=C1C=Cc2ccccc2OC1
O-C-[C;H0;D4;+0:1]1(-[OH;D1;+0:2])-[C:3]=[C:4]-[c:5]:[c:6]-[#8:7]-[C:8]-1>>[O;H0;D1;+0:2]=[C;H0;D3;+0:1]1-[C:3]=[C:4]-[c:5]:[c:6]-[#8:7]-[C:8]-1
45
[{"value": 45.0, "product": "O=C1COC2=C(C=C1)C=C(C=C2)C(=O)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 45.0, "product": "O=C1COC2=C(C=C1)C=C(C=C2)C(=O)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
116 mg (0.54 mmol) of sodium periodate are added at ambient temperature in 4 equal portions, every quarter of an hour, to 135 mg (0.54 mmol) of methyl 3-hydroxy-3-(hydroxymethyl)-2,3-dihydro-1-benzoxepin-7-carboxylate, prepared according to example 45, in solution in 16 ml of a 3/1 dioxane/water mixture. After the usua...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Tertiary alcohol
Ketone
C1=Cc2ccccc2OCC1
C1=Cc2ccccc2OCC1
C1=Cc2ccccc2OCC1
HO-
O1CCOCC1.O
null
null
COC(=O)c1ccc2c(c1)C=CC(O)(CO)CO2>O1CCOCC1.O>COC(=O)c1ccc2c(c1)C=CC(=O)CO2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4bb72300ba5c4c05b76cf13a23b63ef4
COC(=O)c1ccc2c(c1)C=CC(=O)CO2.ClC(Cl)(Cl)Br>>COC(=O)c1ccc2c(c1)C=CC(=C(Cl)Cl)CO2
BrC(Cl)(Cl)Cl.O=C1COC2=C(C=C1)C=C(C=C2)C(=O)OC.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1>>ClC(=C1COC2=C(C=C1)C=C(C=C2)C(=O)OC)Cl
O=[C:13]1[CH:12]=[CH:11][c:9]2[c:8]([cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:10]2)[O:18][CH2:17]1.Cl[C:14](Br)([Cl:15])[Cl:16]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]2[c:9]([cH:10]1)[CH:11]=[CH:12][C:13](=[C:14]([Cl:15])[Cl:16])[CH2:17][O:18]2
COC(=O)c1ccc2c(c1)C=CC(=O)CO2.ClC(Cl)(Cl)Br
COC(=O)c1ccc2c(c1)C=CC(=C(Cl)Cl)CO2
null
null
C(C)#N
C-C Coupling
OtherReaction
5910cf971eb6d9d154a60935a0d4cd400795a28843523ac74cc375ae09a50221
9b69c6acf5f96bd89ba7feda6794a83098e618a606bbf5124735bee2db81e0ee
C=C1C=Cc2ccccc2OC1
Br-[C;H0;D4;+0:1](-Cl)(-[Cl;D1;H0:2])-[Cl;D1;H0:3].O=[C;H0;D3;+0:4]1-[C:5]=[C:6]-[c:7]:[c:8]-[#8:9]-[C:10]-1>>[Cl;D1;H0:2]-[C;H0;D3;+0:1](-[Cl;D1;H0:3])=[C;H0;D3;+0:4]1-[C:5]=[C:6]-[c:7]:[c:8]-[#8:9]-[C:10]-1
74
[{"value": 74.0, "product": "ClC(=C1COC2=C(C=C1)C=C(C=C2)C(=O)OC)Cl", "details": "PERCENTYIELD", "is_desired": false}]
0
CELSIUS
2
HOUR
0.046 ml (2 equivalents) of bromotrichloromethane is added to 50 mg (0.23 mmol) of methyl 3-oxo-2,3-dihydro-1-benzoxepin-7-carboxylate, prepared according to example 49, and 214 mg (0.92 mmol) of triphenylphosphine in suspension in 0.5 ml of acetonitrile, which is stirred beforehand at 0° C. for 2 hours. The reaction m...
10.6084/m9.figshare.5104873.v1
null
Trichloro group.Tertiary halide.Ketone
Alkenyl halide.Alkenyl halide
C1=Cc2ccccc2OCC1
C1=Cc2ccccc2OCC1
C1=Cc2ccccc2OCC1
Br-
C(C)#N
0
2
COC(=O)c1ccc2c(c1)C=CC(=O)CO2.ClC(Cl)(Cl)Br>C(C)#N>COC(=O)c1ccc2c(c1)C=CC(=C(Cl)Cl)CO2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-954ff43e90644cdc809fe4fa5bee8c9a
CN(C)C(=O)c1ccc2c(c1)C=CC(=O)CO2.CNO>>CON=C1C=Cc2cc(C(=O)N(C)C)ccc2OC1
CNO.CN(C(=O)C=1C=CC2=C(C=CC(CO2)=O)C1)C.CO>>CON=C1COC2=C(C=C1)C=C(C=C2)C(=O)N(C)C
O=[C:4]1[CH:5]=[CH:6][c:7]2[cH:8][c:9]([C:10](=[O:11])[N:12]([CH3:13])[CH3:14])[cH:15][cH:16][c:17]2[O:18][CH2:19]1.[CH3:1][NH:3][OH:2]>>[CH3:1][O:2][N:3]=[C:4]1[CH:5]=[CH:6][c:7]2[cH:8][c:9]([C:10](=[O:11])[N:12]([CH3:13])[CH3:14])[cH:15][cH:16][c:17]2[O:18][CH2:19]1
CN(C)C(=O)c1ccc2c(c1)C=CC(=O)CO2.CNO
CON=C1C=Cc2cc(C(=O)N(C)C)ccc2OC1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
5384bfed642291592577e388f462fbe7a47ca7db661aa0250e0927c6c04a2b41
8c052f9ef549b4f361c78f993cdc42cacbd253a7d96709e648aa4ade80c3417e
N=C1C=Cc2ccccc2OC1
O=[C;H0;D3;+0:1]1-[C:2]-[#8:3]-[c:4]:[c:5]-[C:6]=[C:7]-1.[CH3;D1;+0:8]-[NH;D2;+0:9]-[OH;D1;+0:10]>>[CH3;D1;+0:8]-[O;H0;D2;+0:10]-[N;H0;D2;+0:9]=[C;H0;D3;+0:1]1-[C:2]-[#8:3]-[c:4]:[c:5]-[C:6]=[C:7]-1
38
[{"value": 38.0, "product": "CON=C1COC2=C(C=C1)C=C(C=C2)C(=O)N(C)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
37 mg of N-methylhydroxylamine are added to 150 mg (0.65 mmol) of N,N-dimethyl-3-oxo-2,3-dihydro-1-benzoxepin-7-carboxamide, prepared according to example 53, in solution in 1 ml of methanol, and the medium is stirred at ambient temperature for 2 hours. After evaporating the methanol, followed by the conventional treat...
10.6084/m9.figshare.5104873.v1
null
Ketone.Secondary amine
null
C1=Cc2ccccc2OCC1
C1=Cc2ccccc2OCC1
C1=Cc2ccccc2OCC1
HO-
null
null
2
CN(C)C(=O)c1ccc2c(c1)C=CC(=O)CO2.CNO>>CON=C1C=Cc2cc(C(=O)N(C)C)ccc2OC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ec588e9c9ad0476aa2ef0f51fdd2c601
COC(=O)c1ccc2c(c1)C=CC(=CCl)CO2>>O=C(O)c1ccc2c(c1)C=CC(=CCl)CO2
[OH-].[K+].ClC=C1COC2=C(C=C1)C=C(C=C2)C(=O)OC.Cl>>ClC=C1COC2=C(C=C1)C=C(C=C2)C(=O)O
C[O:3][C:2](=[O:1])[c:4]1[cH:5][cH:6][c:7]2[c:8]([cH:9]1)[CH:10]=[CH:11][C:12](=[CH:13][Cl:14])[CH2:15][O:16]2>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][c:7]2[c:8]([cH:9]1)[CH:10]=[CH:11][C:12](=[CH:13][Cl:14])[CH2:15][O:16]2
COC(=O)c1ccc2c(c1)C=CC(=CCl)CO2
O=C(O)c1ccc2c(c1)C=CC(=CCl)CO2
null
null
C(C)O
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
[CH]=C1C=Cc2ccccc2OC1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]
63.4
[{"value": 63.0, "product": "ClC=C1COC2=C(C=C1)C=C(C=C2)C(=O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 63.4, "product": "ClC=C1COC2=C(C=C1)C=C(C=C2)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
145 mg (2.6 mmol) of potassium hydroxide pellets are added to 0.5 g (2 mmol) of methyl 3-(chloromethylene)-2,3-dihydro-1-benzoxepin-7-carboxylate, prepared according to example 32, in solution in 8 ml of 80% aqueous ethanol, and the medium is brought to reflux for 3 hours. After cooling, the medium is brought to acidit...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
C1=Cc2ccccc2OCC1
Other
C(C)O
null
null
COC(=O)c1ccc2c(c1)C=CC(=CCl)CO2>C(C)O>O=C(O)c1ccc2c(c1)C=CC(=CCl)CO2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a0cccb0dc3ef4d53b68c107a8f87a28f
Nc1ccccc1.O=C(O)c1ccc2c(c1)C=CC(=CCl)CO2>>O=C(Nc1ccccc1)c1ccc2c(c1)C=CC(=CCl)CO2
[Cl-].COC1=NC(=NC(=N1)OC)[N+]1(CCOCC1)C.NC1=CC=CC=C1.ClC=C1COC2=C(C=C1)C=C(C=C2)C(=O)O>>ClC=C1COC2=C(C=C1)C=C(C=C2)C(=O)NC2=CC=CC=C2
[NH2:3][c:4]1[cH:5][cH:6][cH:7][cH:8][cH:9]1.O[C:2](=[O:1])[c:10]1[cH:11][cH:12][c:13]2[c:14]([cH:15]1)[CH:16]=[CH:17][C:18](=[CH:19][Cl:20])[CH2:21][O:22]2>>[O:1]=[C:2]([NH:3][c:4]1[cH:5][cH:6][cH:7][cH:8][cH:9]1)[c:10]1[cH:11][cH:12][c:13]2[c:14]([cH:15]1)[CH:16]=[CH:17][C:18](=[CH:19][Cl:20])[CH2:21][O:22]2
Nc1ccccc1.O=C(O)c1ccc2c(c1)C=CC(=CCl)CO2
O=C(Nc1ccccc1)c1ccc2c(c1)C=CC(=CCl)CO2
null
null
CO
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
[CH]=C1C=Cc2cc(C(=O)Nc3ccccc3)ccc2OC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9])-[c:3](:[c:4]):[c:5]
15.3
[{"value": 15.0, "product": "ClC=C1COC2=C(C=C1)C=C(C=C2)C(=O)NC2=CC=CC=C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 15.3, "product": "ClC=C1COC2=C(C=C1)C=C(C=C2)C(=O)NC2=CC=CC=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
127 mg (0.46 mmol) of 4-(4,6-dimethoxy-1,3,5-triazin-2-yl)-4-methylmorpholinium chloride and then 39 mg (0.42 mmol) of aniline are added to 100 mg (0.42 mmol) of 3-(chloromethylene)-2,3-dihydro-1-benzoxepin-7-carboxylic acid, prepared according to example 63, in solution in 4 ml of methanol, and the medium is stirred a...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.C1=Cc2ccccc2OCC1
HO-
CO
null
3
Nc1ccccc1.O=C(O)c1ccc2c(c1)C=CC(=CCl)CO2>CO>O=C(Nc1ccccc1)c1ccc2c(c1)C=CC(=CCl)CO2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-aafb996dd83d4cf1a59f6366ed0cb2bc
COC(=O)c1ccc2c(c1)C=CC(=CCl)CO2>>OCc1ccc2c(c1)C=CC(=CCl)CO2
[H-].C(C(C)C)[Al+]CC(C)C.[Li+].[H-].ClC=C1COC2=C(C=C1)C=C(C=C2)C(=O)OC>>ClC=C1COC2=C(C=C1)C=C(C=C2)CO
CO[C:2](=[O:1])[c:3]1[cH:4][cH:5][c:6]2[c:7]([cH:8]1)[CH:9]=[CH:10][C:11](=[CH:12][Cl:13])[CH2:14][O:15]2>>[OH:1][CH2:2][c:3]1[cH:4][cH:5][c:6]2[c:7]([cH:8]1)[CH:9]=[CH:10][C:11](=[CH:12][Cl:13])[CH2:14][O:15]2
COC(=O)c1ccc2c(c1)C=CC(=CCl)CO2
OCc1ccc2c(c1)C=CC(=CCl)CO2
null
null
ClCCl
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
[CH]=C1C=Cc2ccccc2OC1
C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3](:[c:4]):[c:5]>>[OH;D1;+0:2]-[CH2;D2;+0:1]-[c:3](:[c:4]):[c:5]
108.9
[{"value": 100.0, "product": "ClC=C1COC2=C(C=C1)C=C(C=C2)CO", "details": "PERCENTYIELD", "is_desired": false}, {"value": 108.9, "product": "ClC=C1COC2=C(C=C1)C=C(C=C2)CO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
2.72 ml (2.72 mmol) of a lithium diisobutylaluminum hydride solution are added at a temperature of −78° C. to 217 mg (0.87 mmol) of methyl 3-(chloromethylene)-2,3-dihydro-1-benzoxepin-7-carboxylate, prepared according to example 32, in solution in 10 ml of dichloromethane. The solution is stirred at this temperature fo...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
C1=Cc2ccccc2OCC1
Other
ClCCl
null
1
COC(=O)c1ccc2c(c1)C=CC(=CCl)CO2>ClCCl>OCc1ccc2c(c1)C=CC(=CCl)CO2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c0b09ff6b9044664bc9097945bc3719f
OCc1ccc2c(c1)C=CC(=CCl)CO2>>O=Cc1ccc2c(c1)C=CC(=CCl)CO2
O.C[N+]1(CCOCC1)[O-].ClC=C1COC2=C(C=C1)C=C(C=C2)CO>>ClC=C1COC2=C(C=C1)C=C(C=C2)C=O
[OH:1][CH2:2][c:3]1[cH:4][cH:5][c:6]2[c:7]([cH:8]1)[CH:9]=[CH:10][C:11](=[CH:12][Cl:13])[CH2:14][O:15]2>>[O:1]=[CH:2][c:3]1[cH:4][cH:5][c:6]2[c:7]([cH:8]1)[CH:9]=[CH:10][C:11](=[CH:12][Cl:13])[CH2:14][O:15]2
OCc1ccc2c(c1)C=CC(=CCl)CO2
O=Cc1ccc2c(c1)C=CC(=CCl)CO2
null
[Ru](=O)(=O)(=O)[O-].C(CC)[N+](CCC)(CCC)CCC
ClCCl
Oxidation
Oxidation or Dehydrogenation of Alcohols to Aldehydes and Ketones
41bfa9deea81b465c88ad21fdfb64a2e1ba29490558cf430df132cb98b4a538b
0a03c6724c1862e8f86d4a463afda55b8e067dc6cb42597b472eb7cabc03eda3
[CH]=C1C=Cc2ccccc2OC1
[OH;D1;+0:1]-[CH2;D2;+0:2]-[c:3](:[c:4]):[c:5]>>[O;H0;D1;+0:1]=[CH;D2;+0:2]-[c:3](:[c:4]):[c:5]
76.4
[{"value": 76.0, "product": "ClC=C1COC2=C(C=C1)C=C(C=C2)C=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 76.4, "product": "ClC=C1COC2=C(C=C1)C=C(C=C2)C=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
84 mg (0.62 mmol) of 4-methylmorpholine N-oxide monohydrate and 207 mg of 4 Å molecular sieve are added to 92 mg (0.415 mmol) of [3-(chloromethylene)-2,3-dihydro-1-benzoxepin-7-yl]methanol, prepared according to example 71, in solution in 1 ml of dichloromethane. 14.6 mg (0.041 mmol) of tetrapropylammonium perruthenate...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Aldehyde
null
null
C1=Cc2ccccc2OCC1
null
[Ru](=O)(=O)(=O)[O-].C(CC)[N+](CCC)(CCC)CCC.ClCCl
null
1
OCc1ccc2c(c1)C=CC(=CCl)CO2>[Ru](=O)(=O)(=O)[O-].C(CC)[N+](CCC)(CCC)CCC.ClCCl>O=Cc1ccc2c(c1)C=CC(=CCl)CO2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-68307f44708f49ae8a56e3c5e7660de9
NO.O=Cc1ccc2c(c1)C=CC(=CCl)CO2>>CC(=NO)c1ccc2c(c1)C=CC(=CCl)CO2
C(C)(=O)[O-].[Na+].Cl.NO.ClC=C1COC2=C(C=C1)C=C(C=C2)C=O>>ClC=C1COC2=C(C=C1)C=C(C=C2)C(C)=NO
[NH2:3][OH:4].O=[CH:2][c:5]1[cH:6][cH:7][c:8]2[c:9]([cH:10]1)[CH:11]=[CH:12][C:13](=[CH:14][Cl:15])[CH2:16][O:17]2>>[CH3:1][C:2](=[N:3][OH:4])[c:5]1[cH:6][cH:7][c:8]2[c:9]([cH:10]1)[CH:11]=[CH:12][C:13](=[CH:14][Cl:15])[CH2:16][O:17]2
NO.O=Cc1ccc2c(c1)C=CC(=CCl)CO2
CC(=NO)c1ccc2c(c1)C=CC(=CCl)CO2
null
null
CO
Heteroatom Alkylation and Arylation
OtherReaction
26f32c058bcc6b69b34e9c38433bccb165270e0a55ab24439c783c1aee9d8dac
3593c4a8dedbac5f92a1a749cef37ecd686935362f91b9154f0c9930a5edea38
[CH]=C1C=Cc2ccccc2OC1
O=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4].[NH2;D1;+0:5]-[O;D1;H1:6]>>[C;D1;H3:7]-[C;H0;D3;+0:1](=[N;H0;D2;+0:5]-[O;D1;H1:6])-[c:2](:[c:3]):[c:4]
103.1
[{"value": 100.0, "product": "ClC=C1COC2=C(C=C1)C=C(C=C2)C(C)=NO", "details": "PERCENTYIELD", "is_desired": false}, {"value": 103.1, "product": "ClC=C1COC2=C(C=C1)C=C(C=C2)C(C)=NO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
24
HOUR
12.3 mg (0.15 mmol) of sodium acetate and then 10.4 mg (0.15 mmol) of hydroxylamine hydrochloride are added at ambient temperature to 30 mg (0.136 mmol) of 3-(chloromethylene)-2,3-dihydro-1-benzoxepin-7-carbaldehyde, prepared according to example 72, in solution in 2 ml of methanol. The solution is stirred for 24 hours...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Primary amine
Oxime
null
null
C1=Cc2ccccc2OCC1
null
CO
null
24
NO.O=Cc1ccc2c(c1)C=CC(=CCl)CO2>CO>CC(=NO)c1ccc2c(c1)C=CC(=CCl)CO2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c0e13ba0b93e45088f5ce0a2dc8c4dcf
CC1(CCC[P+](c2ccccc2)(c2ccccc2)c2ccccc2)OCCO1.O=Cc1ccc2c(c1)C=CC(=CCl)CO2>>CC1(CCC=Cc2ccc3c(c2)C=CC(=CCl)CO3)OCCO1
C(CCC)[Li].[I-].CC1(OCCO1)CCC[P+](C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1.O.ClC=C1COC2=C(C=C1)C=C(C=C2)C=O>>ClC=C1COC2=C(C=C1)C=C(C=C2)C=CCCC2(OCCO2)C
c1ccc([P+](c2ccccc2)(c2ccccc2)[CH2:5][CH2:4][CH2:3][C:2]2([CH3:1])[O:20][CH2:21][CH2:22][O:23]2)cc1.O=[CH:6][c:7]1[cH:8][cH:9][c:10]2[c:11]([cH:12]1)[CH:13]=[CH:14][C:15](=[CH:16][Cl:17])[CH2:18][O:19]2>>[CH3:1][C:2]1([CH2:3][CH2:4][CH:5]=[CH:6][c:7]2[cH:8][cH:9][c:10]3[c:11]([cH:12]2)[CH:13]=[CH:14][C:15](=[CH:16][Cl:...
CC1(CCC[P+](c2ccccc2)(c2ccccc2)c2ccccc2)OCCO1.O=Cc1ccc2c(c1)C=CC(=CCl)CO2
CC1(CCC=Cc2ccc3c(c2)C=CC(=CCl)CO3)OCCO1
null
null
O1CCCC1.ClCCl
C-C Coupling
Wittig with Phosphonium
cb5f277ac55a0e763ef643becc05f1522019cc4161daceb249ed2d634b78153b
cedc9d4b791e43eacf8e7ecfa6a98d1dc0438794e96e4f1c4bef436b78f82bd8
[CH]=C1C=Cc2cc(C=CCCC3OCCO3)ccc2OC1
O=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4].[C:5]-[C:6]-[CH2;D2;+0:7]-[P+](-c1:c:c:c:c:c:1)(-c1:c:c:c:c:c:1)-c1:c:c:c:c:c:1>>[C:5]-[C:6]-[CH;D2;+0:7]=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4]
71
[{"value": 71.0, "product": "ClC=C1COC2=C(C=C1)C=C(C=C2)C=CCCC2(OCCO2)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 64.2, "product": "ClC=C1COC2=C(C=C1)C=C(C=C2)C=CCCC2(OCCO2)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
1
HOUR
0.206 ml (0.41 mmol) of a 1.9M n-butyllithium solution is added dropwise to 207 mg (0.435 mmol) of [3-(2-methyl-1,3-dioxolan-2-yl)propyl](triphenyl)phosphonium iodide in suspension in 3.2 ml of tetrahydrofuran cooled to 0° C. The medium is stirred for one hour and then the ylide is added at 0° C., via a hollow tube, to...
10.6084/m9.figshare.5104873.v1
null
Aldehyde
null
c1ccccc1.c1ccccc1.c1ccccc1
null
C1=Cc2ccccc2OCC1.C1COCO1
HO-
O1CCCC1.ClCCl
0
1
CC1(CCC[P+](c2ccccc2)(c2ccccc2)c2ccccc2)OCCO1.O=Cc1ccc2c(c1)C=CC(=CCl)CO2>O1CCCC1.ClCCl>CC1(CCC=Cc2ccc3c(c2)C=CC(=CCl)CO3)OCCO1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5c3c7961006b41ffb02668b7da8d8836
CC1(CCC=Cc2ccc3c(c2)C=CC(=CCl)CO3)OCCO1>>CC(=O)CCC=Cc1ccc2c(c1)C=CC(=CCl)CO2
ClC=C1COC2=C(C=C1)C=C(C=C2)C=CCCC2(OCCO2)C.CC(=O)C.C1(=CC=C(C=C1)S(=O)(=O)O)C>>ClC=C1COC2=C(C=C1)C=C(C=C2)C=CCCC(C)=O
C1C[O:3][C:2]([CH3:1])([CH2:4][CH2:5][CH:6]=[CH:7][c:8]2[cH:9][cH:10][c:11]3[c:12]([cH:13]2)[CH:14]=[CH:15][C:16](=[CH:17][Cl:18])[CH2:19][O:20]3)O1>>[CH3:1][C:2](=[O:3])[CH2:4][CH2:5][CH:6]=[CH:7][c:8]1[cH:9][cH:10][c:11]2[c:12]([cH:13]1)[CH:14]=[CH:15][C:16](=[CH:17][Cl:18])[CH2:19][O:20]2
CC1(CCC=Cc2ccc3c(c2)C=CC(=CCl)CO3)OCCO1
CC(=O)CCC=Cc1ccc2c(c1)C=CC(=CCl)CO2
null
CC#N.CC#N.Cl[Pd]Cl
ClCCl
Miscellaneous
Ketal hydrolysis to ketone
bc99a45944d6d67c8bd263755d04463b42623d20ce36570ebfd14e405f44ca50
547697208447432e865290cf95eed8e4fcddc12f59856b7ddbf24dc1accb1210
[CH]=C1C=Cc2ccccc2OC1
[C:1]=[C:2]-[C:3]-[C:4]-[C;H0;D4;+0:5]1(-[C;D1;H3:6])-O-C-C-[O;H0;D2;+0:7]-1>>[C:1]=[C:2]-[C:3]-[C:4]-[C;H0;D3;+0:5](-[C;D1;H3:6])=[O;H0;D1;+0:7]
80.4
[{"value": 80.0, "product": "ClC=C1COC2=C(C=C1)C=C(C=C2)C=CCCC(C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 80.4, "product": "ClC=C1COC2=C(C=C1)C=C(C=C2)C=CCCC(C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
6 mg (0.023 mmol) of bis(acetonitrile)palladium(II) chloride are added to 79 mg (0.237 mmol) of 3-(chloromethylene)-7-[4-(2-methyl-1,3-dioxolan-2-yl)-1-butenyl]-2,3-dihydro-1-benzoxepin, prepared according to example 74, in solution in 1.5 ml of dichloromethane. After stirring at ambient temperature for 3 hours, 0.5 ml...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether
Ketone
C1COCO1
null
C1=Cc2ccccc2OCC1
HO-
CC#N.CC#N.Cl[Pd]Cl.ClCCl
null
3
CC1(CCC=Cc2ccc3c(c2)C=CC(=CCl)CO3)OCCO1>CC#N.CC#N.Cl[Pd]Cl.ClCCl>CC(=O)CCC=Cc1ccc2c(c1)C=CC(=CCl)CO2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d42fe0218dfb4682b7e7b0388106e575
C=C(CCl)CCl.CC(=O)c1ccc(O)c(C=O)c1>>C=C(CCl)COc1ccc(C(C)=O)cc1C=O
Cl.C([O-])([O-])=O.[Na+].[Na+].ClCC(=C)CCl.C(C)(=O)C=1C=CC(=C(C=O)C1)O>>C(C)(=O)C=1C=CC(=C(C=O)C1)OCC(=C)CCl
Cl[CH2:5][C:2](=[CH2:1])[CH2:3][Cl:4].[OH:6][c:7]1[cH:8][cH:9][c:10]([C:11]([CH3:12])=[O:13])[cH:14][c:15]1[CH:16]=[O:17]>>[CH2:1]=[C:2]([CH2:3][Cl:4])[CH2:5][O:6][c:7]1[cH:8][cH:9][c:10]([C:11]([CH3:12])=[O:13])[cH:14][c:15]1[CH:16]=[O:17]
C=C(CCl)CCl.CC(=O)c1ccc(O)c(C=O)c1
C=C(CCl)COc1ccc(C(C)=O)cc1C=O
null
[I-].C(CCC)[N+](CCCC)(CCCC)CCCC
O.CN(C=O)C
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
7e1040116e3a4cf0e8ec5cc7865388d9cd0efabce6d320a1c25a36e411018d8b
d5f4610d46ccc0478471c5bc0fb862644eaf764bbc5d93badb39d54f6ec8e0a5
c1ccccc1
Cl-[CH2;D2;+0:1]-[C:2](-[C:3])=[C;D1;H2:4].[O;D1;H0:5]=[C:6]-[c:7]:[c:8](-[OH;D1;+0:9]):[c:10]>>[C:3]-[C:2](=[C;D1;H2:4])-[CH2;D2;+0:1]-[O;H0;D2;+0:9]-[c:8](:[c:10]):[c:7]-[C:6]=[O;D1;H0:5]
52.7
[{"value": 52.0, "product": "C(C)(=O)C=1C=CC(=C(C=O)C1)OCC(=C)CCl", "details": "PERCENTYIELD", "is_desired": false}, {"value": 52.7, "product": "C(C)(=O)C=1C=CC(=C(C=O)C1)OCC(=C)CCl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
21
HOUR
6.02 g (16.31 mmol) of tetrabutylammonium iodide, 6.17 g (2.5 equivalents) of sodium carbonate and, finally, 6.7 ml (58.2 mmol) of 2-chloromethyl-3-chloro-1-propene are successively added to 3.82 g (23 mmol) of 5-acetyl-2-hydroxybenzaldehyde, prepared according to Tromelin, A. et al., Synthesis, (1985), 1074–1076, and ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic alcohol
Ether
null
null
c1ccccc1
HCl
[I-].C(CCC)[N+](CCCC)(CCCC)CCCC.O.CN(C=O)C
null
21
C=C(CCl)CCl.CC(=O)c1ccc(O)c(C=O)c1>[I-].C(CCC)[N+](CCCC)(CCCC)CCCC.O.CN(C=O)C>C=C(CCl)COc1ccc(C(C)=O)cc1C=O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-74898563749d45e290e940e012a4e69f
C=C(CCl)COc1ccc(C(C)=O)cc1C=O.[I-]>>C=C(CI)COc1ccc(C(C)=O)cc1C=O
[I-].[Na+].C(C)(=O)C=1C=CC(=C(C=O)C1)OCC(=C)CCl.O>>C(C)(=O)C=1C=CC(=C(C=O)C1)OCC(=C)CI
Cl[CH2:3][C:2](=[CH2:1])[CH2:5][O:6][c:7]1[cH:8][cH:9][c:10]([C:11]([CH3:12])=[O:13])[cH:14][c:15]1[CH:16]=[O:17].[I-:4]>>[CH2:1]=[C:2]([CH2:3][I:4])[CH2:5][O:6][c:7]1[cH:8][cH:9][c:10]([C:11]([CH3:12])=[O:13])[cH:14][c:15]1[CH:16]=[O:17]
C=C(CCl)COc1ccc(C(C)=O)cc1C=O.[I-]
C=C(CI)COc1ccc(C(C)=O)cc1C=O
null
null
CC(=O)C
Functional Group Interconversion
OtherReaction
e944a2acb95a43a23818321f2ac2f96ba2f2b8d34f52c1cfd1e3802d2403177f
e2ca6f9fe1078a3836d617896a4e5cc310fb155ca459b021e2b549b3e61f1df7
c1ccccc1
Cl-[CH2;D2;+0:1]-[C:2](-[C:3])=[C;D1;H2:4].[I-;H0;D0:5]>>[C:3]-[C:2](=[C;D1;H2:4])-[CH2;D2;+0:1]-[I;H0;D1;+0:5]
100.1
[{"value": 100.0, "product": "C(C)(=O)C=1C=CC(=C(C=O)C1)OCC(=C)CI", "details": "PERCENTYIELD", "is_desired": false}, {"value": 100.1, "product": "C(C)(=O)C=1C=CC(=C(C=O)C1)OCC(=C)CI", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
5
HOUR
531 mg (3.54 mmol) of sodium iodide are added to 894 mg (3.54 mmol) of 5-acetyl-2-{[2-(chloromethyl)-2-propenyl]oxy}benzaldehyde in solution in 10 ml of distilled acetone. The medium is brought to reflux and is stirred for 5 hours. Water is added and then the solution is concentrated. After the addition of water and di...
10.6084/m9.figshare.5104873.v1
null
Primary halide
Primary halide
null
null
c1ccccc1
Other
CC(=O)C
null
5
C=C(CCl)COc1ccc(C(C)=O)cc1C=O.[I-]>CC(=O)C>C=C(CI)COc1ccc(C(C)=O)cc1C=O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-790f5a2328ca4e0baebd073feb8f231d
C=C(CI)COc1ccc(C(C)=O)cc1C=O>>C=C1C=Cc2cc(C(C)=O)ccc2OC1
C[O-].[Na+].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C(C)(=O)C=1C=CC(=C(C=O)C1)OCC(=C)CI.O>>C=C1COC2=C(C=C1)C=C(C=C2)C(C)=O
O=[CH:4][c:5]1[cH:6][c:7]([C:8]([CH3:9])=[O:10])[cH:11][cH:12][c:13]1[O:14][CH2:15][C:2](=[CH2:1])[CH2:3]I>>[CH2:1]=[C:2]1[CH:3]=[CH:4][c:5]2[cH:6][c:7]([C:8]([CH3:9])=[O:10])[cH:11][cH:12][c:13]2[O:14][CH2:15]1
C=C(CI)COc1ccc(C(C)=O)cc1C=O
C=C1C=Cc2cc(C(C)=O)ccc2OC1
null
null
C(C)#N.CO
C-C Coupling
OtherReaction
cd8aa2006e08ebd6c5752a804163d33604e551cb274de5cfef9b1f643743b122
a3dca447376ff0c6fe3968bb1ab0785c8926c417c53ba2b61f8ebdb52a7e5a2a
C=C1C=Cc2ccccc2OC1
I-[CH2;D2;+0:1]-[C:2](-[C:3])=[C;D1;H2:4].O=[CH;D2;+0:5]-[c:6](:[c:7]):[c:8]>>[C:3]-[C:2](=[C;D1;H2:4])-[CH;D2;+0:1]=[CH;D2;+0:5]-[c:6](:[c:7]):[c:8]
58
[{"value": 58.0, "product": "C=C1COC2=C(C=C1)C=C(C=C2)C(C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 57.9, "product": "C=C1COC2=C(C=C1)C=C(C=C2)C(C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
14
HOUR
973 mg (3.575 mmol) of triphenylphosphine are added under argon to 1.118 g (3.25 mmol) of 5-acetyl-2-{[2-(iodomethyl)-2-propenyl]oxy}benzaldehyde in solution in 30 ml of acetonitrile. The medium is brought to reflux and is stirred for 14 hours. After cooling the solution, 0.743 ml (3.25 mmol) of a 25% solution of sodiu...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aldehyde
null
null
C1=Cc2ccccc2OCC1
C1=Cc2ccccc2OCC1
HI
C(C)#N.CO
null
14
C=C(CI)COc1ccc(C(C)=O)cc1C=O>C(C)#N.CO>C=C1C=Cc2cc(C(C)=O)ccc2OC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-3b79389c3e42424d85f643dbd66bbb59
CC(=O)c1ccc2c(c1)C=CC(=O)CO2.ClC[P+](c1ccccc1)(c1ccccc1)c1ccccc1>>CC(=O)c1ccc2c(c1)C=CC(=CCl)CO2
C(CCC)[Li].[Cl-].ClC[P+](C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1.C(C)(=O)C=1C=CC2=C(C=CC(CO2)=O)C1>>ClC=C1COC2=C(C=C1)C=C(C=C2)C(C)=O
O=[C:12]1[CH:11]=[CH:10][c:8]2[c:7]([cH:6][cH:5][c:4]([C:2]([CH3:1])=[O:3])[cH:9]2)[O:16][CH2:15]1.c1ccc([P+](c2ccccc2)(c2ccccc2)[CH2:13][Cl:14])cc1>>[CH3:1][C:2](=[O:3])[c:4]1[cH:5][cH:6][c:7]2[c:8]([cH:9]1)[CH:10]=[CH:11][C:12](=[CH:13][Cl:14])[CH2:15][O:16]2
CC(=O)c1ccc2c(c1)C=CC(=O)CO2.ClC[P+](c1ccccc1)(c1ccccc1)c1ccccc1
CC(=O)c1ccc2c(c1)C=CC(=CCl)CO2
null
null
O1CCCC1.CCCCC
C-C Coupling
Wittig with Phosphonium
539d98d0a68c79c0ce64fb9b77faf88c2e8998170a817390f2eb321da849bd7d
4ccc953afa1928fe5ef55f22a0c593e017875730e9bc8868efb0bd3550ea5ba6
[CH]=C1C=Cc2ccccc2OC1
O=[C;H0;D3;+0:1]1-[C:2]=[C:3]-[c:4]:[c:5]-[#8:6]-[C:7]-1.[Cl;D1;H0:8]-[CH2;D2;+0:9]-[P+](-c1:c:c:c:c:c:1)(-c1:c:c:c:c:c:1)-c1:c:c:c:c:c:1>>[Cl;D1;H0:8]-[CH;D2;+0:9]=[C;H0;D3;+0:1]1-[C:2]=[C:3]-[c:4]:[c:5]-[#8:6]-[C:7]-1
55
[{"value": 55.0, "product": "ClC=C1COC2=C(C=C1)C=C(C=C2)C(C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 55.0, "product": "ClC=C1COC2=C(C=C1)C=C(C=C2)C(C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
1
HOUR
1.1 equivalents of n-butyllithium are added to 309 mg (0.89 mmol) of chloromethyltriphenylphosphonium chloride in 5 ml of tetrahydrofuran cooled to 0° C. After stirring for one hour, 150 mg (0.74 mmol) of 7-acetyl-1-benzoxepin-3(2H)-one, prepared according to example 79, are added at ambient temperature. The medium is ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ketone
null
C1=Cc2ccccc2OCC1.c1ccccc1.c1ccccc1.c1ccccc1
C1=Cc2ccccc2OCC1
C1=Cc2ccccc2OCC1
HO-
O1CCCC1.CCCCC
0
1
CC(=O)c1ccc2c(c1)C=CC(=O)CO2.ClC[P+](c1ccccc1)(c1ccccc1)c1ccccc1>O1CCCC1.CCCCC>CC(=O)c1ccc2c(c1)C=CC(=CCl)CO2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-fc7c84b695ff493b9d788642c9763ea0
Cc1ccc(O)cc1.O=[N+]([O-])c1cccc(S(=O)(=O)Cl)c1>>Cc1ccc(OS(=O)(=O)c2cccc(N)c2)cc1
[Sn](Cl)Cl.C1=CC(=CC=C1O)C.N1=CC=CC=C1.[N+](=O)([O-])C=1C=C(C=CC1)S(=O)(=O)Cl>>NC=1C=C(C=CC1)S(=O)(=O)OC1=CC=C(C=C1)C
[CH3:1][c:2]1[cH:3][cH:4][c:5]([OH:6])[cH:17][cH:18]1.O=[N+:15]([O-])[c:14]1[cH:13][cH:12][cH:11][c:10]([S:7](Cl)(=[O:8])=[O:9])[cH:16]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([O:6][S:7](=[O:8])(=[O:9])[c:10]2[cH:11][cH:12][cH:13][c:14]([NH2:15])[cH:16]2)[cH:17][cH:18]1
Cc1ccc(O)cc1.O=[N+]([O-])c1cccc(S(=O)(=O)Cl)c1
Cc1ccc(OS(=O)(=O)c2cccc(N)c2)cc1
null
null
Cl.C(Cl)(Cl)Cl
Acylation
OtherReaction
0f17f52386aa31153b43ba6292c0360cf635a875b254cd05f4597231d283adc0
5452d749a309ee3a24f18a5d8d8ac3d612b02da20bfd045c9772626370a17052
O=S(=O)(Oc1ccccc1)c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]:[c:7](-[N+;H0;D3:8](=O)-[O-]):[c:9].[OH;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[NH2;D1;+0:8]-[c:7](:[c:9]):[c:6]:[c:4](-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[O;H0;D2;+0:10]-[c:11](:[c:12]):[c:13]):[c:5]
71.4
[{"value": 71.4, "product": "NC=1C=C(C=CC1)S(=O)(=O)OC1=CC=C(C=C1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
To 50 g (0.463 mole) of p-cresol (4-methylphenol) and 37 mL (0.458 mole) of pyridine dissolved in 250 mL of chloroform was added 50 g (0.226 mole) of 3-nitrobenzenesulfonyl chloride. The reaction was allowed to stir at ambient temperature. After 2 hours, the reaction was judged complete by TLC and the volatiles were re...
10.6084/m9.figshare.5104873.v1
null
Nitro group.Aromatic alcohol.Sulfonyl halide
Primary amine.Sulfonate
null
null
c1ccccc1.c1ccccc1
Other
Cl.C(Cl)(Cl)Cl
null
2
Cc1ccc(O)cc1.O=[N+]([O-])c1cccc(S(=O)(=O)Cl)c1>Cl.C(Cl)(Cl)Cl>Cc1ccc(OS(=O)(=O)c2cccc(N)c2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-cfbc990807b743f29b14ef279f7a239c
Cc1ccc(OS(=O)(=O)c2cccc(NS(=O)(=O)c3ccc4ccc(NC(=O)Nc5ccc6ccc(S(=O)(=O)O)cc6c5)cc4c3)c2)cc1.[OH-]>>O=C(Nc1ccc2ccc(S(=O)(=O)[O-])cc2c1)Nc1ccc2ccc(S(=O)(=O)Nc3cccc(S(=O)(=O)O)c3)cc2c1.O=C(Nc1ccc2ccc(S(=O)(=O)[O-])cc2c1)Nc1ccc2ccc(S(=O)(=O)Nc3cccc(S(=O)(=O)O)c3)cc2c1.[Na+]
CC1=CC=C(C=C1)OS(=O)(=O)C=1C=C(C=CC1)NS(=O)(=O)C1=CC=C2C=CC(=CC2=C1)NC(=O)NC1=CC=C2C=CC(=CC2=C1)S(=O)(=O)O.[OH-].[Na+].Cl>>[Na+].[Na+].S(=O)(=O)(O)C=1C=C(C=CC1)NS(=O)(=O)C1=CC=C2C=CC(=CC2=C1)NC(=O)NC1=CC=C2C=CC(=CC2=C1)S(=O)(=O)[O-].S(=O)(=O)(O)C=1C=C(C=CC1)NS(=O)(=O)C1=CC=C2C=CC(=CC2=C1)NC(=O)NC1=CC=C2C=CC(=CC2=C1)S(=...
[O:1]=[S:68](=[O:37])([c:67]1[cH:66][cH:65][c:64]2[cH:63][cH:62][c:61]([NH:60][C:44]([NH:3][c:2]3[cH:20][cH:21][c:22]4[cH:8][cH:9][c:10]([S:11](=[O:12])(=[O:13])[OH:14])[cH:15][c:41]4[cH:40]3)=[O:43])[cH:84][c:83]2[cH:82]1)[NH:71][c:72]1[cH:73][cH:74][cH:75][c:76]([S:77]([O:56][c:46]2[cH:4][cH:51][c:52]([CH3:57])[cH:58...
Cc1ccc(OS(=O)(=O)c2cccc(NS(=O)(=O)c3ccc4ccc(NC(=O)Nc5ccc6ccc(S(=O)(=O)O)cc6c5)cc4c3)c2)cc1.[OH-]
O=C(Nc1ccc2ccc(S(=O)(=O)[O-])cc2c1)Nc1ccc2ccc(S(=O)(=O)Nc3cccc(S(=O)(=O)O)c3)cc2c1.O=C(Nc1ccc2ccc(S(=O)(=O)[O-])cc2c1)Nc1ccc2ccc(S(=O)(=O)Nc3cccc(S(=O)(=O)O)c3)cc2c1.[Na+]
null
null
null
Aromatic Heterocycle Formation
OtherReaction
2dd1ba3fff9c92dc787cca5101038606519bf17e25df652cde93905c3989c0e0
2ed33179e64b4d883ef533a708ed0330b53fffe689f52713ef507e3428d8d94b
O=C(Nc1ccc2ccccc2c1)Nc1ccc2ccc(S(=O)(=O)Nc3ccccc3)cc2c1.O=C(Nc1ccc2ccccc2c1)Nc1ccc2ccc(S(=O)(=O)Nc3ccccc3)cc2c1
[CH3;D1;+0:1]-[c;H0;D3;+0:2]1:[cH;D2;+0:3]:[cH;D2;+0:4]:[c;H0;D3;+0:5](-[O;H0;D2;+0:6]-[S;H0;D4;+0:7](=[O;D1;H0:8])(=[O;H0;D1;+0:9])-[c:10](:[c:11]):[c:12]:[c:13]-[#7:14]-[S;H0;D4;+0:15](=[O;H0;D1;+0:16])(=[O;H0;D1;+0:17])-[c:18](:[c:19]):[c:20]):[c:21]:[cH;D2;+0:22]:1.[O;D1;H0:23]=[#16:24](=[O;D1;H0:25])(-[OH;D1;+0:26...
null
[]
null
null
6
HOUR
To 8 mg (0.011 mmol) of compound 8 was added 2 mL of 5 N NaOH. The reaction was allowed to stir at ambient temperature for 6 hours. The reaction was acidified with 6 N HCl and the solution was added to a small reverse-phase (C18) solid phase extraction column. The column was washed with H2O followed by 50:50 (v:v) CH3C...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Urea.Sulfonate
Sulfonamide.Sulfonamide.Urea.Urea.Sulfonic acid.Sulfonic acid.Sulfonic acid
c1ccc2ccccc2c1.c1ccccc1
c1ccc2ccccc2c1.c1ccc2ccccc2c1.c1ccccc1.c1ccc2ccccc2c1
c1ccc2ccccc2c1.c1ccc2ccccc2c1.c1ccccc1.c1ccc2ccccc2c1.c1ccc2ccccc2c1.c1ccccc1
null
null
null
6
Cc1ccc(OS(=O)(=O)c2cccc(NS(=O)(=O)c3ccc4ccc(NC(=O)Nc5ccc6ccc(S(=O)(=O)O)cc6c5)cc4c3)c2)cc1.[OH-]>>O=C(Nc1ccc2ccc(S(=O)(=O)[O-])cc2c1)Nc1ccc2ccc(S(=O)(=O)Nc3cccc(S(=O)(=O)O)c3)cc2c1.O=C(Nc1ccc2ccc(S(=O)(=O)[O-])cc2c1)Nc1ccc2ccc(S(=O)(=O)Nc3cccc(S(=O)(=O)O)c3)cc2c1.[Na+]
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d8f8941d558d487dac6430f9c8d0c26d
Cc1ccc(OS(=O)(=O)c2cccc(NS(=O)(=O)c3ccc4ccc(NC(=O)Nc5ccc6ccc(S(=O)(=O)Nc7cccc(S(=O)(=O)Oc8ccc(C)cc8)c7)cc6c5)cc4c3)c2)cc1.[OH-]>>O=C(Nc1ccc2ccc(S(=O)(=O)Nc3cccc(S(=O)(=O)[O-])c3)cc2c1)Nc1ccc2ccc(S(=O)(=O)Nc3cccc(S(=O)(=O)O)c3)cc2c1.O=C(Nc1ccc2ccc(S(=O)(=O)Nc3cccc(S(=O)(=O)[O-])c3)cc2c1)Nc1ccc2ccc(S(=O)(=O)Nc3cccc(S(=O)...
CC1=CC=C(C=C1)OS(=O)(=O)C=1C=C(C=CC1)NS(=O)(=O)C1=CC=C2C=CC(=CC2=C1)NC(=O)NC1=CC=C2C=CC(=CC2=C1)S(=O)(=O)NC=1C=C(C=CC1)S(=O)(=O)OC1=CC=C(C=C1)C.[OH-].[Na+].Cl>>[Na+].[Na+].S(=O)(=O)(O)C=1C=C(C=CC1)NS(=O)(=O)C1=CC=C2C=CC(=CC2=C1)NC(=O)NC1=CC=C2C=CC(=CC2=C1)S(=O)(=O)NC=1C=C(C=CC1)S(=O)(=O)[O-].S(=O)(=O)(O)C=1C=C(C=CC1)NS...
[O:1]=[C:2]([NH:3][c:81]1[cH:82][cH:83][c:84]2[cH:85][cH:86][c:87]([S:88](=[O:89])(=[O:90])[NH:91][c:92]3[cH:93][cH:94][cH:95][c:96]([S:36](=[O:37])(=[O:38])[O:75][c:67]4[cH:68][cH:34][c:35]([CH3:50])[cH:71][cH:76]4)[cH:101]3)[cH:102][c:103]2[cH:104]1)[NH:55][c:56]1[cH:57][cH:58][c:59]2[cH:8][cH:9][c:10]([S:11](=[O:12]...
Cc1ccc(OS(=O)(=O)c2cccc(NS(=O)(=O)c3ccc4ccc(NC(=O)Nc5ccc6ccc(S(=O)(=O)Nc7cccc(S(=O)(=O)Oc8ccc(C)cc8)c7)cc6c5)cc4c3)c2)cc1.[OH-]
O=C(Nc1ccc2ccc(S(=O)(=O)Nc3cccc(S(=O)(=O)[O-])c3)cc2c1)Nc1ccc2ccc(S(=O)(=O)Nc3cccc(S(=O)(=O)O)c3)cc2c1.O=C(Nc1ccc2ccc(S(=O)(=O)Nc3cccc(S(=O)(=O)[O-])c3)cc2c1)Nc1ccc2ccc(S(=O)(=O)Nc3cccc(S(=O)(=O)O)c3)cc2c1.[Na+]
null
null
null
Aromatic Heterocycle Formation
OtherReaction
ec5c62283bf6a54bc73e468b3adbdbc87f44856eea1662142f34da2be77d6851
4cd607b55decb7cd9e62b5940d4bb0492ea6857d4bf00321865fbff3b89163be
O=C(Nc1ccc2ccc(S(=O)(=O)Nc3ccccc3)cc2c1)Nc1ccc2ccc(S(=O)(=O)Nc3ccccc3)cc2c1.O=C(Nc1ccc2ccc(S(=O)(=O)Nc3ccccc3)cc2c1)Nc1ccc2ccc(S(=O)(=O)Nc3ccccc3)cc2c1
[CH3;D1;+0:1]-[c;H0;D3;+0:2]1:[cH;D2;+0:3]:[cH;D2;+0:4]:[c;H0;D3;+0:5](-[O;H0;D2;+0:6]-[S;H0;D4;+0:7](=[O;D1;H0:8])(=[O;D1;H0:9])-[c;H0;D3;+0:10](:[c:11]:[c:12]):[c:13]:[c:14]):[c:15]:[cH;D2;+0:16]:1.[CH3;D1;+0:17]-[c;H0;D3;+0:18]1:[c:19]:[cH;D2;+0:20]:[c;H0;D3;+0:21](-[O;H0;D2;+0:22]-[#16:23](=[O;D1;H0:24])(=[O;D1;H0:...
null
[]
null
null
6
HOUR
To 35 mg (0.036 mmol) of compound 9 was added 2 mL of 5 N NaOH. The reaction was allowed to stir at ambient temperature for 6 hours. The reaction was acidified with 6 N HCl and the solution was added to a small reverse-phase (C18) solid phase extraction column. The column was washed with H2O followed by 50:50 (v:v) CH3...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Urea.Sulfonate
Sulfonamide.Sulfonamide.Sulfonamide.Urea.Urea.Sulfonic acid.Sulfonic acid.Sulfonic acid
c1ccc2ccccc2c1.c1ccccc1.c1ccccc1.c1ccc2ccccc2c1.c1ccccc1
c1ccc2ccccc2c1.c1ccc2ccccc2c1.c1ccccc1.c1ccc2ccccc2c1.c1ccccc1.c1ccc2ccccc2c1.c1ccccc1
c1ccc2ccccc2c1.c1ccccc1.c1ccc2ccccc2c1.c1ccccc1.c1ccc2ccccc2c1.c1ccccc1.c1ccc2ccccc2c1.c1ccccc1
null
null
null
6
Cc1ccc(OS(=O)(=O)c2cccc(NS(=O)(=O)c3ccc4ccc(NC(=O)Nc5ccc6ccc(S(=O)(=O)Nc7cccc(S(=O)(=O)Oc8ccc(C)cc8)c7)cc6c5)cc4c3)c2)cc1.[OH-]>>O=C(Nc1ccc2ccc(S(=O)(=O)Nc3cccc(S(=O)(=O)[O-])c3)cc2c1)Nc1ccc2ccc(S(=O)(=O)Nc3cccc(S(=O)(=O)O)c3)cc2c1.O=C(Nc1ccc2ccc(S(=O)(=O)Nc3cccc(S(=O)(=O)[O-])c3)cc2c1)Nc1ccc2ccc(S(=O)(=O)Nc3cccc(S(=O)...
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a9e74391cbf14242bd3b427717f72d39
Cc1ccc(OS(=O)(=O)c2cccc(NS(=O)(=O)c3cc(O)c4ccc(NC(=O)Nc5ccc6c(O)cc(S(=O)(=O)O)cc6c5)cc4c3)c2)cc1.O=C(Nc1ccc2ccc(S(=O)(=O)[O-])cc2c1)Nc1ccc2ccc(S(=O)(=O)Nc3cccc(S(=O)(=O)O)c3)cc2c1>>O=C(Nc1ccc2c(O)cc(S(=O)(=O)O)cc2c1)Nc1ccc2c(O)cc(S(=O)(=O)Nc3cccc(S(=O)(=O)O)c3)cc2c1
OC1=CC(=CC2=CC(=CC=C12)NC(=O)NC1=CC2=CC(=CC(=C2C=C1)O)S(=O)(=O)NC1=CC(=CC=C1)S(=O)(=O)OC1=CC=C(C=C1)C)S(=O)(=O)O.[Na+].[Na+].S(=O)(=O)(O)C=1C=C(C=CC1)NS(=O)(=O)C1=CC=C2C=CC(=CC2=C1)NC(=O)NC1=CC=C2C=CC(=CC2=C1)S(=O)(=O)[O-].S(=O)(=O)(O)C=1C=C(C=CC1)NS(=O)(=O)C1=CC=C2C=CC(=CC2=C1)NC(=O)NC1=CC=C2C=CC(=CC2=C1)S(=O)(=O)[O-]...
Cc1ccc(O[S:37]([c:36]2[cH:35][cH:34][cH:33][c:32]([NH:31][S:28]([c:27]3[cH:26][c:24]([OH:25])[c:23]4[cH:22][cH:21][c:20]([NH:19][C:2](=[O:1])[NH:3][c:4]5[cH:5][cH:6][c:7]6[c:8]([OH:9])[cH:10][c:11]([S:12](=[O:13])(=[O:14])[OH:15])[cH:16][c:17]6[cH:18]5)[cH:44][c:43]4[cH:42]3)(=[O:29])=[O:30])[cH:41]2)(=[O:38])=[O:39])c...
Cc1ccc(OS(=O)(=O)c2cccc(NS(=O)(=O)c3cc(O)c4ccc(NC(=O)Nc5ccc6c(O)cc(S(=O)(=O)O)cc6c5)cc4c3)c2)cc1.O=C(Nc1ccc2ccc(S(=O)(=O)[O-])cc2c1)Nc1ccc2ccc(S(=O)(=O)Nc3cccc(S(=O)(=O)O)c3)cc2c1
O=C(Nc1ccc2c(O)cc(S(=O)(=O)O)cc2c1)Nc1ccc2c(O)cc(S(=O)(=O)Nc3cccc(S(=O)(=O)O)c3)cc2c1
null
null
null
Miscellaneous
OtherReaction
5651ad236e30fc5e1fb136f94e6b47964049343b023233af6edbbb99ad9da079
c29fbd699f0e9548504fd648142985b754dd32ed818b292df8b8b9a4b9bc07ea
O=C(Nc1ccc2ccccc2c1)Nc1ccc2ccc(S(=O)(=O)Nc3ccccc3)cc2c1
C-c1:c:c:c(-O-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6]):c:c:1.O=C(-N-c1:c:c:c2:c:c:c(-S(=O)(=O)-[O-]):c:c:2:c:1)-N-c1:c:c:c2:c:c:c(-S(=O)(=O)-N-c3:c:c:c:c(-S(=O)(=O)-[OH;D1;+0:7]):c:3):c:c:2:c:1>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[OH;D1;+0:7])-[c:4](:[c:5]):[c:6]
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This compound was prepared from compound 10 according to the procedure described for the synthesis of compound 12. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
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Sulfonamide.Urea.Sulfonic acid.Sulfonic acid.Sulfonate
Sulfonic acid
c1ccccc1.c1ccc2ccccc2c1.c1ccc2ccccc2c1.c1ccccc1
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c1ccc2ccccc2c1.c1ccc2ccccc2c1.c1ccccc1
HO-
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Cc1ccc(OS(=O)(=O)c2cccc(NS(=O)(=O)c3cc(O)c4ccc(NC(=O)Nc5ccc6c(O)cc(S(=O)(=O)O)cc6c5)cc4c3)c2)cc1.O=C(Nc1ccc2ccc(S(=O)(=O)[O-])cc2c1)Nc1ccc2ccc(S(=O)(=O)Nc3cccc(S(=O)(=O)O)c3)cc2c1>>O=C(Nc1ccc2c(O)cc(S(=O)(=O)O)cc2c1)Nc1ccc2c(O)cc(S(=O)(=O)Nc3cccc(S(=O)(=O)O)c3)cc2c1