dataset_id
large_stringclasses
414 values
reaction_id
large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
reactant_smiles
large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-23d8b3aa860946449b836e743b5e5189
Brc1ccc2c(ccn2Cc2ccccc2)c1.OB(O)c1ccccc1>>c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
C(C1=CC=CC=C1)N1C=CC2=CC(=CC=C12)Br.ClCCl.C([O-])([O-])=O.[K+].[K+].C1(=CC=CC=C1)B(O)O>>C(C1=CC=CC=C1)N1C=CC2=CC(=CC=C12)C1=CC=CC=C1
Br[c:11]1[cH:10][c:9]2[cH:8][cH:7][n:6]([CH2:5][c:4]3[cH:3][cH:2][cH:1][cH:22][cH:21]3)[c:20]2[cH:19][cH:18]1.OB(O)[c:12]1[cH:13][cH:14][cH:15][cH:16][cH:17]1>>[cH:1]1[cH:2][cH:3][c:4]([CH2:5][n:6]2[cH:7][cH:8][c:9]3[cH:10][c:11](-[c:12]4[cH:13][cH:14][cH:15][cH:16][cH:17]4)[cH:18][cH:19][c:20]23)[cH:21][cH:22]1
Brc1ccc2c(ccn2Cc2ccccc2)c1.OB(O)c1ccccc1
c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
null
C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.Cl[Pd]Cl.[Fe+2]
O1CCOCC1.O
C-C Coupling
Suzuki coupling with boronic acids
42e21206f0250bb469664981cf521bd21ce6ff7bf8a8e9271f94397f7d3b79cb
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](:[#7;a:5]):[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[#7;a:5]:[c:4]1:[c:6]:[c:7]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]):[c:2]:[c:3]:1
35
[{"value": 35.0, "product": "C(C1=CC=CC=C1)N1C=CC2=CC(=CC=C12)C1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 34.5, "product": "C(C1=CC=CC=C1)N1C=CC2=CC(=CC=C12)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
1-Benzyl-5-phenyl-1H-indole was prepared by coupling 1-benzyl-5-bromo-1H-indole (2.72 g, 9.50 mmol), and phenylboronic acid (1.39 g, 11.4 mmol), using [1,1′-bis(diphenylphosphino)ferrocene]dichloropalladium (II) complex with dichloromethane (1:1) (0.266 g, 0.326 mmol), and potassium carbonate (2.06 g, 14.9 mmol) in dio...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccccc1.c1ccc2[nH]ccc2c1.c1ccccc1
HBr.B
C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.Cl[Pd]Cl.[Fe+2].O1CCOCC1.O
null
null
Brc1ccc2c(ccn2Cc2ccccc2)c1.OB(O)c1ccccc1>C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.C1=CC=C(C=C1)P([C-]2C=CC=C2)C3=CC=CC=C3.Cl[Pd]Cl.[Fe+2].O1CCOCC1.O>c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-137b44c12907427ba89083a530a22b08
CCO.O=C(Cl)C(=O)Cl.c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1>>CCOC(=O)C(=O)c1cn(Cc2ccccc2)c2ccc(-c3ccccc3)cc12
C(C1=CC=CC=C1)N1C=CC2=CC(=CC=C12)C1=CC=CC=C1.C(C(=O)Cl)(=O)Cl.C(C)O>>C(C1=CC=CC=C1)N1C=C(C2=CC(=CC=C12)C1=CC=CC=C1)C(C(=O)OCC)=O
[CH3:1][CH2:2][OH:3].Cl[C:4](=[O:5])[C:6](Cl)=[O:7].[cH:8]1[cH:9][n:10]([CH2:11][c:12]2[cH:13][cH:14][cH:15][cH:16][cH:17]2)[c:18]2[cH:19][cH:20][c:21](-[c:22]3[cH:23][cH:24][cH:25][cH:26][cH:27]3)[cH:28][c:29]12>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[C:6](=[O:7])[c:8]1[cH:9][n:10]([CH2:11][c:12]2[cH:13][cH:14][cH:15][cH:16...
CCO.O=C(Cl)C(=O)Cl.c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
CCOC(=O)C(=O)c1cn(Cc2ccccc2)c2ccc(-c3ccccc3)cc12
null
null
null
C-C Coupling
OtherReaction
e42beb79999369525e781f5f2a8c25a764f237d2f2302bca9902d8152413d7f2
b36dbf7958ca5ae3ba65aceed13fac6c31bf5a9975134271733ce2a3346931a4
c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C;H0;D3;+0:3](-Cl)=[O;D1;H0:4].[C;D1;H3:5]-[C:6]-[OH;D1;+0:7].[C:8]-[#7;a:9]1:[c:10]:[cH;D2;+0:11]:[c:12](:[c:13]):[c:14]:1:[c:15]>>[C:8]-[#7;a:9]1:[c:10]:[c;H0;D3;+0:11](-[C;H0;D3;+0:3](=[O;D1;H0:4])-[C;H0;D3;+0:1](=[O;D1;H0:2])-[O;H0;D2;+0:7]-[C:6]-[C;D1;H3:5]):[c:12](:[c:13]):[c:14]:...
66
[{"value": 66.0, "product": "C(C1=CC=CC=C1)N1C=C(C2=CC(=CC=C12)C1=CC=CC=C1)C(C(=O)OCC)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
Ethyl {1-benzyl-5-phenyl-1H-indol-3-yl}(oxo)acetate was prepared from 1-benzyl-5-phenyl-1H-indole (0.846 g, 2.99 mmol), oxalyl chloride (0.78 mL, 9.0 mmol), and ethanol (2 mL), following the procedure described in Step 3 of Example 1. Purification by flash chromatography (Biotage apparatus) using 5-7.5% ethyl acetate i...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Acyl halide.Primary alcohol
Ketone.Ester
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
c1ccccc1.c1ccc2[nH]ccc2c1.c1ccccc1
HCl
null
null
null
CCO.O=C(Cl)C(=O)Cl.c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1>>CCOC(=O)C(=O)c1cn(Cc2ccccc2)c2ccc(-c3ccccc3)cc12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c63258f45f3848609e0a8ea5042f1287
CCOC(=O)C(=O)c1cn(Cc2ccccc2)c2ccc(-c3ccccc3)cc12>>O=C(O)C(=O)c1cn(Cc2ccccc2)c2ccc(-c3ccccc3)cc12
C(C1=CC=CC=C1)N1C=C(C2=CC(=CC=C12)C1=CC=CC=C1)C(C(=O)OCC)=O.[OH-].[K+]>>C(C1=CC=CC=C1)N1C=C(C2=CC(=CC=C12)C1=CC=CC=C1)C(C(=O)O)=O
CC[O:3][C:2](=[O:1])[C:4](=[O:5])[c:6]1[cH:7][n:8]([CH2:9][c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[c:16]2[cH:17][cH:18][c:19](-[c:20]3[cH:21][cH:22][cH:23][cH:24][cH:25]3)[cH:26][c:27]12>>[O:1]=[C:2]([OH:3])[C:4](=[O:5])[c:6]1[cH:7][n:8]([CH2:9][c:10]2[cH:11][cH:12][cH:13][cH:14][cH:15]2)[c:16]2[cH:17][cH:18][c:19]...
CCOC(=O)C(=O)c1cn(Cc2ccccc2)c2ccc(-c3ccccc3)cc12
O=C(O)C(=O)c1cn(Cc2ccccc2)c2ccc(-c3ccccc3)cc12
null
null
O.C1CCOC1
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[C:4](=[O;D1;H0:5])-[c:6]:[c:7]:[#7;a:8]>>[#7;a:8]:[c:7]:[c:6]-[C:4](=[O;D1;H0:5])-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
62.3
[{"value": 62.0, "product": "C(C1=CC=CC=C1)N1C=C(C2=CC(=CC=C12)C1=CC=CC=C1)C(C(=O)O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 62.3, "product": "C(C1=CC=CC=C1)N1C=C(C2=CC(=CC=C12)C1=CC=CC=C1)C(C(=O)O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
{1-Benzyl-5-phenyl-1H-indol-3-yl}(oxo)acetic acid was prepared from ethyl {1-benzyl-5-phenyl-1H-indol-3-yl}(oxo)acetate (0.680 g, 1.77 mmol), and potassium hydroxide (0.322 g, 5.74 mmol) in THF (10 mL) and water (10 mL), following the procedure described in Step 4 of Example 5. Crystallization from acetonitrile, and dr...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccc2[nH]ccc2c1.c1ccccc1
Other
O.C1CCOC1
null
null
CCOC(=O)C(=O)c1cn(Cc2ccccc2)c2ccc(-c3ccccc3)cc12>O.C1CCOC1>O=C(O)C(=O)c1cn(Cc2ccccc2)c2ccc(-c3ccccc3)cc12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-83ac8374c5154999b98d4a40fefbd012
Brc1ccc2[nH]ccc2c1.Cc1ccc(CBr)cc1>>Cc1ccc(Cn2ccc3cc(Br)ccc32)cc1
[H-].[Na+].BrC=1C=C2C=CNC2=CC1.CC1=CC=C(CBr)C=C1>>BrC=1C=C2C=CN(C2=CC1)CC1=CC=C(C=C1)C
[nH:7]1[cH:8][cH:9][c:10]2[cH:11][c:12]([Br:13])[cH:14][cH:15][c:16]12.Br[CH2:6][c:5]1[cH:4][cH:3][c:2]([CH3:1])[cH:18][cH:17]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([CH2:6][n:7]2[cH:8][cH:9][c:10]3[cH:11][c:12]([Br:13])[cH:14][cH:15][c:16]23)[cH:17][cH:18]1
Brc1ccc2[nH]ccc2c1.Cc1ccc(CBr)cc1
Cc1ccc(Cn2ccc3cc(Br)ccc32)cc1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
92cc004fc3e2a92f5c9aa0385cdf93f1126e35d5aa485f4f5fe9240c9543c8fe
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ccc(Cn2ccc3ccccc32)cc1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[c:5]:[c:6]1:[c:7]:[c:8]:[c:9]:[nH;D2;+0:10]:1>>[c:5]:[c:6]1:[c:7]:[c:8]:[c:9]:[n;H0;D3;+0:10]:1-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
1
HOUR
NaH (60%, 2.53 g, 63.1 mmol) was added portionwise to a stirring solution of 5-bromoindole (8.25 g, 42.1 mmol) in DMF (80 mL) at 0° C. under a nitrogen atmosphere over a period of 10 min. The mixture was then warmed up to room temperature. After the reaction mixture was stirred at room temperature for 1 hour, 4-methylb...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
c1ccccc1.c1ccc2[nH]ccc2c1
HBr
CN(C)C=O
null
1
Brc1ccc2[nH]ccc2c1.Cc1ccc(CBr)cc1>CN(C)C=O>Cc1ccc(Cn2ccc3cc(Br)ccc32)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c8100daffee34b4a9962e3d643e03b3a
Cc1ccc(Cn2ccc3cc(Br)ccc32)cc1.OB(O)c1ccccc1>>Cc1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
BrC=1C=C2C=CN(C2=CC1)CC1=CC=C(C=C1)C.C1(=CC=CC=C1)B(O)O.C([O-])([O-])=O.[K+].[K+].C(Cl)Cl>>CC1=CC=C(CN2C=CC3=CC(=CC=C23)C2=CC=CC=C2)C=C1
Br[c:12]1[cH:11][c:10]2[cH:9][cH:8][n:7]([CH2:6][c:5]3[cH:4][cH:3][c:2]([CH3:1])[cH:23][cH:22]3)[c:21]2[cH:20][cH:19]1.OB(O)[c:13]1[cH:14][cH:15][cH:16][cH:17][cH:18]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([CH2:6][n:7]2[cH:8][cH:9][c:10]3[cH:11][c:12](-[c:13]4[cH:14][cH:15][cH:16][cH:17][cH:18]4)[cH:19][cH:20][c:21]23)[cH:22...
Cc1ccc(Cn2ccc3cc(Br)ccc32)cc1.OB(O)c1ccccc1
Cc1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
null
null
O.O1CCOCC1.O
C-C Coupling
Suzuki coupling with boronic acids
42e21206f0250bb469664981cf521bd21ce6ff7bf8a8e9271f94397f7d3b79cb
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](:[#7;a:5]):[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[#7;a:5]:[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]):[c:7]:[c:6]:1
49
[{"value": 49.0, "product": "CC1=CC=C(CN2C=CC3=CC(=CC=C23)C2=CC=CC=C2)C=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 48.5, "product": "CC1=CC=C(CN2C=CC3=CC(=CC=C23)C2=CC=CC=C2)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
70
CELSIUS
2
DAY
A mixture of 5-bromo-1-(4-methylbenzyl)-1H-indole (1.0 g, 3.33 mmol), benzeneboronic acid (0.621 g, 5.0 mmol), potassium carbonate (0.691 g, 5.0 mmol), and [1′1′-bis(diphenylphosphino)-ferrocene]dichloropalladium(II) complex with methylenechloride (1:1) (0.816 g, 1.0 mmol) in dioxane-water (10:1, 16.5 mL) was stirred a...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccccc1.c1ccc2[nH]ccc2c1.c1ccccc1
HBr.B
O.O1CCOCC1.O
70
48
Cc1ccc(Cn2ccc3cc(Br)ccc32)cc1.OB(O)c1ccccc1>O.O1CCOCC1.O>Cc1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5e7bd16ba5f94b02b3b6a3c660acd8af
Cc1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1.O=C(Cl)C(=O)Cl>>Cc1ccc(Cn2cc(C(=O)C(=O)O)c3cc(-c4ccccc4)ccc32)cc1
C(C(=O)Cl)(=O)Cl.CC1=CC=C(CN2C=CC3=CC(=CC=C23)C2=CC=CC=C2)C=C1.C1CCOC1>>CC1=CC=C(CN2C=C(C3=CC(=CC=C23)C2=CC=CC=C2)C(C(=O)O)=O)C=C1
[CH3:1][c:2]1[cH:3][cH:4][c:5]([CH2:6][n:7]2[cH:8][cH:9][c:15]3[cH:16][c:17](-[c:18]4[cH:19][cH:20][cH:21][cH:22][cH:23]4)[cH:24][cH:25][c:26]23)[cH:27][cH:28]1.Cl[C:10](=[O:11])[C:12](Cl)=[O:13]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([CH2:6][n:7]2[cH:8][c:9]([C:10](=[O:11])[C:12](=[O:13])[OH:14])[c:15]3[cH:16][c:17](-[c:18]4...
Cc1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1.O=C(Cl)C(=O)Cl
Cc1ccc(Cn2cc(C(=O)C(=O)O)c3cc(-c4ccccc4)ccc32)cc1
null
null
null
Acylation
OtherReaction
9d127b05b36fe9fe6fc80547d3614a823e90d1399390b2ba6617beb8202d8432
6b048b617f07704989b0d7eff26dc61c44694ea4e42b339d6d7680e8458e5255
c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C;H0;D3;+0:3](-Cl)=[O;D1;H0:4].[C:5]-[#7;a:6]1:[c:7]:[cH;D2;+0:8]:[c:9](:[c:10]):[c:11]:1:[c:12]>>[C:5]-[#7;a:6]1:[c:7]:[c;H0;D3;+0:8](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C;H0;D3;+0:3](=[O;D1;H0:4])-[O;D1;H1:13]):[c:9](:[c:10]):[c:11]:1:[c:12]
72
[{"value": 72.0, "product": "CC1=CC=C(CN2C=C(C3=CC(=CC=C23)C2=CC=CC=C2)C(C(=O)O)=O)C=C1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
Oxalyl chloride (0.474 mL, 5.43 mmol) was added dropwise to a stirring solution of 1-(4-methylbenzyl)-5-phenyl-1H-indole (0.46 g, 1.55 mmol) in THF (15 mL) at room temperature over a period of 5 minutes under a nitrogen atmosphere. After the reaction mixture was stirred at room temperature for 4 hours, the reaction was...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Acyl halide
Carboxylic acid.Ketone
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
c1ccccc1.c1ccc2[nH]ccc2c1.c1ccccc1
Other
null
null
4
Cc1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1.O=C(Cl)C(=O)Cl>>Cc1ccc(Cn2cc(C(=O)C(=O)O)c3cc(-c4ccccc4)ccc32)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f9b1ebdd05e34c87bf371a2dd67ee2c3
Cc1ccc(Cn2ccc3cc(Br)ccc32)cc1.OB(O)c1ccc(OC(F)(F)F)cc1>>Cc1ccc(Cn2ccc3cc(-c4ccc(OC(F)(F)F)cc4)ccc32)cc1
BrC=1C=C2C=CN(C2=CC1)CC1=CC=C(C=C1)C.FC(OC1=CC=C(C=C1)B(O)O)(F)F>>CC1=CC=C(CN2C=CC3=CC(=CC=C23)C2=CC=C(C=C2)OC(F)(F)F)C=C1
Br[c:12]1[cH:11][c:10]2[cH:9][cH:8][n:7]([CH2:6][c:5]3[cH:4][cH:3][c:2]([CH3:1])[cH:28][cH:27]3)[c:26]2[cH:25][cH:24]1.OB(O)[c:13]1[cH:14][cH:15][c:16]([O:17][C:18]([F:19])([F:20])[F:21])[cH:22][cH:23]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([CH2:6][n:7]2[cH:8][cH:9][c:10]3[cH:11][c:12](-[c:13]4[cH:14][cH:15][c:16]([O:17][C:1...
Cc1ccc(Cn2ccc3cc(Br)ccc32)cc1.OB(O)c1ccc(OC(F)(F)F)cc1
Cc1ccc(Cn2ccc3cc(-c4ccc(OC(F)(F)F)cc4)ccc32)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
42e21206f0250bb469664981cf521bd21ce6ff7bf8a8e9271f94397f7d3b79cb
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](:[#7;a:5]):[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[#7;a:5]:[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]):[c:7]:[c:6]:1
null
[]
null
null
null
null
The title compound was prepared from 5-bromo-1-(4-methylbenzyl)-1H-indole (Step 1 of Example 25) and 4-(trifluoromethoxy)phenylboronic acid in substantially the same manner, as described in Step 2 of Example 25. The product was obtained as an oil. Mass spectrum (ESI, [M+H]+) m/z 382. 1HNMR (300 MHz, DMSO-d6): δ 7.83 (s...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccccc1.c1ccc2[nH]ccc2c1.c1ccccc1
HBr.B
null
null
null
Cc1ccc(Cn2ccc3cc(Br)ccc32)cc1.OB(O)c1ccc(OC(F)(F)F)cc1>>Cc1ccc(Cn2ccc3cc(-c4ccc(OC(F)(F)F)cc4)ccc32)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f4f94b3fac1948a2b4bd89a4f06f205a
Brc1ccc2[nH]ccc2c1.Fc1ccc(CBr)cc1>>Fc1ccc(Cn2ccc3cc(Br)ccc32)cc1
FC1=CC=C(CBr)C=C1.BrC=1C=C2C=CNC2=CC1>>BrC=1C=C2C=CN(C2=CC1)CC1=CC=C(C=C1)F
[nH:7]1[cH:8][cH:9][c:10]2[cH:11][c:12]([Br:13])[cH:14][cH:15][c:16]12.Br[CH2:6][c:5]1[cH:4][cH:3][c:2]([F:1])[cH:18][cH:17]1>>[F:1][c:2]1[cH:3][cH:4][c:5]([CH2:6][n:7]2[cH:8][cH:9][c:10]3[cH:11][c:12]([Br:13])[cH:14][cH:15][c:16]23)[cH:17][cH:18]1
Brc1ccc2[nH]ccc2c1.Fc1ccc(CBr)cc1
Fc1ccc(Cn2ccc3cc(Br)ccc32)cc1
null
null
null
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
92cc004fc3e2a92f5c9aa0385cdf93f1126e35d5aa485f4f5fe9240c9543c8fe
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ccc(Cn2ccc3ccccc32)cc1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[c:5]:[c:6]1:[c:7]:[c:8]:[c:9]:[nH;D2;+0:10]:1>>[c:5]:[c:6]1:[c:7]:[c:8]:[c:9]:[n;H0;D3;+0:10]:1-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
The title compound was prepared from 4-fluorobenzyl bromide and 5-bromoindole in substantially the same manner, as described in Step 1 of Example 25. The product was obtained as a white solid; mp: 57-58° C. Mass spectrum (APCI, [M+H]+) m/z 304. 1 HNMR (400 MHz, DMSO-d6): δ 7.73 (d, 1H, J=1.8 Hz), 7.55 (d, 1H, J=3.2 Hz)...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
c1ccccc1.c1ccc2[nH]ccc2c1
HBr
null
null
null
Brc1ccc2[nH]ccc2c1.Fc1ccc(CBr)cc1>>Fc1ccc(Cn2ccc3cc(Br)ccc32)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-1a929905409f4df2874edb2ef39fb252
Fc1ccc(Cn2ccc3cc(Br)ccc32)cc1.OB(O)c1ccc(OC(F)(F)F)cc1>>Fc1ccc(Cn2ccc3cc(-c4ccc(OC(F)(F)F)cc4)ccc32)cc1
BrC=1C=C2C=CN(C2=CC1)CC1=CC=C(C=C1)F.FC(OC1=CC=C(C=C1)B(O)O)(F)F>>FC1=CC=C(CN2C=CC3=CC(=CC=C23)C2=CC=C(C=C2)OC(F)(F)F)C=C1
Br[c:12]1[cH:11][c:10]2[cH:9][cH:8][n:7]([CH2:6][c:5]3[cH:4][cH:3][c:2]([F:1])[cH:28][cH:27]3)[c:26]2[cH:25][cH:24]1.OB(O)[c:13]1[cH:14][cH:15][c:16]([O:17][C:18]([F:19])([F:20])[F:21])[cH:22][cH:23]1>>[F:1][c:2]1[cH:3][cH:4][c:5]([CH2:6][n:7]2[cH:8][cH:9][c:10]3[cH:11][c:12](-[c:13]4[cH:14][cH:15][c:16]([O:17][C:18]([...
Fc1ccc(Cn2ccc3cc(Br)ccc32)cc1.OB(O)c1ccc(OC(F)(F)F)cc1
Fc1ccc(Cn2ccc3cc(-c4ccc(OC(F)(F)F)cc4)ccc32)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
42e21206f0250bb469664981cf521bd21ce6ff7bf8a8e9271f94397f7d3b79cb
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](:[#7;a:5]):[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[#7;a:5]:[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]):[c:7]:[c:6]:1
null
[]
null
null
null
null
The title compound was prepared from 5-bromo-1-(4-fluorobenzyl)-1H-indole and 4-(trifluoromethoxy)phenylboronic acid in substantially the same manner, as described in Step 2 of Example 25. The product was obtained as an oil. Mass spectrum (ESI, [M+H]+) m/z 386. 1HNMR (300 MHz, DMSO-d6): δ 7.84 (s, 1H), 7.76 (d, 2H, J=8...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccccc1.c1ccc2[nH]ccc2c1.c1ccccc1
HBr.B
null
null
null
Fc1ccc(Cn2ccc3cc(Br)ccc32)cc1.OB(O)c1ccc(OC(F)(F)F)cc1>>Fc1ccc(Cn2ccc3cc(-c4ccc(OC(F)(F)F)cc4)ccc32)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-879c708c3c7d4ea29f1ee08d3d08a6d4
Fc1ccc(Cn2ccc3cc(Br)ccc32)cc1.OB(O)c1ccccc1>>Fc1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
BrC=1C=C2C=CN(C2=CC1)CC1=CC=C(C=C1)F.C1(=CC=CC=C1)B(O)O>>FC1=CC=C(CN2C=CC3=CC(=CC=C23)C2=CC=CC=C2)C=C1
Br[c:12]1[cH:11][c:10]2[cH:9][cH:8][n:7]([CH2:6][c:5]3[cH:4][cH:3][c:2]([F:1])[cH:23][cH:22]3)[c:21]2[cH:20][cH:19]1.OB(O)[c:13]1[cH:14][cH:15][cH:16][cH:17][cH:18]1>>[F:1][c:2]1[cH:3][cH:4][c:5]([CH2:6][n:7]2[cH:8][cH:9][c:10]3[cH:11][c:12](-[c:13]4[cH:14][cH:15][cH:16][cH:17][cH:18]4)[cH:19][cH:20][c:21]23)[cH:22][cH...
Fc1ccc(Cn2ccc3cc(Br)ccc32)cc1.OB(O)c1ccccc1
Fc1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
42e21206f0250bb469664981cf521bd21ce6ff7bf8a8e9271f94397f7d3b79cb
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](:[#7;a:5]):[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[#7;a:5]:[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]):[c:7]:[c:6]:1
null
[]
null
null
null
null
The title compound was prepared from 5-bromo-1-(4-fluorobenzyl)-1H-indole (Step 1 of Example 27) and benzeneboronic acid in substantially the same manner, as described in Step 2 of Example 25. The product was obtained as an oil. Mass spectrum (ESI, [M+H]+) m/z 302. 1HNMR (300 MHz, DMSO-d6): δ 7.81 (s, 1H), 7.63 (d, 2H,...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccccc1.c1ccc2[nH]ccc2c1.c1ccccc1
HBr.B
null
null
null
Fc1ccc(Cn2ccc3cc(Br)ccc32)cc1.OB(O)c1ccccc1>>Fc1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-8c462a37513741d69cfce9855fa61341
Brc1ccc2[nH]ccc2c1.CCCCBr>>CCCCn1ccc2cc(Br)ccc21
BrCCCC.BrC=1C=C2C=CNC2=CC1>>BrC=1C=C2C=CN(C2=CC1)CCCC
[nH:5]1[cH:6][cH:7][c:8]2[cH:9][c:10]([Br:11])[cH:12][cH:13][c:14]12.Br[CH2:4][CH2:3][CH2:2][CH3:1]>>[CH3:1][CH2:2][CH2:3][CH2:4][n:5]1[cH:6][cH:7][c:8]2[cH:9][c:10]([Br:11])[cH:12][cH:13][c:14]12
Brc1ccc2[nH]ccc2c1.CCCCBr
CCCCn1ccc2cc(Br)ccc21
null
null
null
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
92cc004fc3e2a92f5c9aa0385cdf93f1126e35d5aa485f4f5fe9240c9543c8fe
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ccc2[nH]ccc2c1
Br-[CH2;D2;+0:1]-[C:2]-[C:3].[c:4]:[c:5]1:[c:6]:[c:7]:[c:8]:[nH;D2;+0:9]:1>>[C:3]-[C:2]-[CH2;D2;+0:1]-[n;H0;D3;+0:9]1:[c:8]:[c:7]:[c:6]:[c:5]:1:[c:4]
null
[]
null
null
null
null
The title compound was prepared from 1-bromobutane (11 mL, 101 mmol) and 5-bromoindole (20 g, 101 mmol) in substantially the same manner, as described in Step 1 of Example 25. The product was obtained as an oil. Mass spectrum (ESI, [M+H]+) m/z 252. 1HNMR (300 MHz, DMSO-d6): δ 7.71 (d, 1H, J=1.9 Hz), 7.46 (d, 1H, J=8.7 ...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
HBr
null
null
null
Brc1ccc2[nH]ccc2c1.CCCCBr>>CCCCn1ccc2cc(Br)ccc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-916330ebdd15492aaf890057b09b7397
CCCCn1ccc2cc(Br)ccc21.OB(O)c1ccc(Cl)cc1>>CCCCn1ccc2cc(-c3ccc(Cl)cc3)ccc21
BrC=1C=C2C=CN(C2=CC1)CCCC.ClC1=CC=C(C=C1)B(O)O>>C(CCC)N1C=CC2=CC(=CC=C12)C1=CC=C(C=C1)Cl
Br[c:10]1[cH:9][c:8]2[cH:7][cH:6][n:5]([CH2:4][CH2:3][CH2:2][CH3:1])[c:20]2[cH:19][cH:18]1.OB(O)[c:11]1[cH:12][cH:13][c:14]([Cl:15])[cH:16][cH:17]1>>[CH3:1][CH2:2][CH2:3][CH2:4][n:5]1[cH:6][cH:7][c:8]2[cH:9][c:10](-[c:11]3[cH:12][cH:13][c:14]([Cl:15])[cH:16][cH:17]3)[cH:18][cH:19][c:20]12
CCCCn1ccc2cc(Br)ccc21.OB(O)c1ccc(Cl)cc1
CCCCn1ccc2cc(-c3ccc(Cl)cc3)ccc21
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
42e21206f0250bb469664981cf521bd21ce6ff7bf8a8e9271f94397f7d3b79cb
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc3[nH]ccc3c2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](:[#7;a:5]):[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[#7;a:5]:[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]):[c:7]:[c:6]:1
null
[]
null
null
null
null
The title compound was prepared from 5-bromo-1-butyl-1H-indole and 4-chlorophenylboronic acid in substantially the same manner, as described in Step 2 of Example 25. The product was obtained as an oil. Mass spectrum (ESI, [M+H]+) m/z 284. 1HNMR (400 MHz, DMSO-d6): δ 7.81 (s, 1H), 7.67 (d, 2H, J=8.56 Hz), 7.54 (d, 1H, J...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1
HBr.B
null
null
null
CCCCn1ccc2cc(Br)ccc21.OB(O)c1ccc(Cl)cc1>>CCCCn1ccc2cc(-c3ccc(Cl)cc3)ccc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-26f7f0c637c0454d8a1d2894c49931ac
CCCCn1ccc2cc(Br)ccc21.OB(O)c1cccc(Cl)c1>>CCCCn1ccc2cc(-c3cccc(Cl)c3)ccc21
BrC=1C=C2C=CN(C2=CC1)CCCC.ClC=1C=C(C=CC1)B(O)O>>C(CCC)N1C=CC2=CC(=CC=C12)C1=CC(=CC=C1)Cl
Br[c:10]1[cH:9][c:8]2[cH:7][cH:6][n:5]([CH2:4][CH2:3][CH2:2][CH3:1])[c:20]2[cH:19][cH:18]1.OB(O)[c:11]1[cH:12][cH:13][cH:14][c:15]([Cl:16])[cH:17]1>>[CH3:1][CH2:2][CH2:3][CH2:4][n:5]1[cH:6][cH:7][c:8]2[cH:9][c:10](-[c:11]3[cH:12][cH:13][cH:14][c:15]([Cl:16])[cH:17]3)[cH:18][cH:19][c:20]12
CCCCn1ccc2cc(Br)ccc21.OB(O)c1cccc(Cl)c1
CCCCn1ccc2cc(-c3cccc(Cl)c3)ccc21
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
42e21206f0250bb469664981cf521bd21ce6ff7bf8a8e9271f94397f7d3b79cb
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc3[nH]ccc3c2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](:[#7;a:5]):[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[#7;a:5]:[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]):[c:7]:[c:6]:1
null
[]
null
null
null
null
The title compound was prepared from 5-bromo-1-butyl-1H-indole (Step 1 of Example 29) and 3-chlorophenylboronic acid in substantially the same manner, as described in Step 2 of Example 25. The product was obtained as an oil. Mass spectrum (APCI, [M+H]+) m/z 284. 1HNMR (400 MHz, DMSO-d6): δ 7.85 (s, 1H), 7.69 (s, 1H), 7...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1
HBr.B
null
null
null
CCCCn1ccc2cc(Br)ccc21.OB(O)c1cccc(Cl)c1>>CCCCn1ccc2cc(-c3cccc(Cl)c3)ccc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-cced9169477847a6bc9e85b61cea955c
CCCCn1ccc2cc(Br)ccc21.COc1cccc(B(O)O)c1>>CCCCn1ccc2cc(-c3cccc(OC)c3)ccc21
BrC=1C=C2C=CN(C2=CC1)CCCC.COC=1C=C(C=CC1)B(O)O>>C(CCC)N1C=CC2=CC(=CC=C12)C1=CC(=CC=C1)OC
Br[c:10]1[cH:9][c:8]2[cH:7][cH:6][n:5]([CH2:4][CH2:3][CH2:2][CH3:1])[c:21]2[cH:20][cH:19]1.OB(O)[c:11]1[cH:12][cH:13][cH:14][c:15]([O:16][CH3:17])[cH:18]1>>[CH3:1][CH2:2][CH2:3][CH2:4][n:5]1[cH:6][cH:7][c:8]2[cH:9][c:10](-[c:11]3[cH:12][cH:13][cH:14][c:15]([O:16][CH3:17])[cH:18]3)[cH:19][cH:20][c:21]12
CCCCn1ccc2cc(Br)ccc21.COc1cccc(B(O)O)c1
CCCCn1ccc2cc(-c3cccc(OC)c3)ccc21
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
42e21206f0250bb469664981cf521bd21ce6ff7bf8a8e9271f94397f7d3b79cb
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc3[nH]ccc3c2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](:[#7;a:5]):[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[#7;a:5]:[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]):[c:7]:[c:6]:1
null
[]
null
null
null
null
The title compound was prepared from 5-bromo-1-butyl-1H-indole (Step 1 of Example 29) and 3-methoxyphenylboronic acid in substantially the same manner, as described in Step 2 of Example 25. The product was obtained as an oil. Mass spectrum (APCI, [M+H]+) m/z 280. 1HNMR (300 MHz, DMSO-d6): δ 7.81 (s, 1H), 7.52 (d, 1H, J...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1
HBr.B
null
null
null
CCCCn1ccc2cc(Br)ccc21.COc1cccc(B(O)O)c1>>CCCCn1ccc2cc(-c3cccc(OC)c3)ccc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0c32c86514d84644a64ee65e2a0d2648
CCCCn1ccc2cc(Br)ccc21.COc1ccc(B(O)O)cc1>>CCCCn1ccc2cc(-c3ccc(OC)cc3)ccc21
BrC=1C=C2C=CN(C2=CC1)CCCC.COC1=CC=C(C=C1)B(O)O>>C(CCC)N1C=CC2=CC(=CC=C12)C1=CC=C(C=C1)OC
Br[c:10]1[cH:9][c:8]2[cH:7][cH:6][n:5]([CH2:4][CH2:3][CH2:2][CH3:1])[c:21]2[cH:20][cH:19]1.OB(O)[c:11]1[cH:12][cH:13][c:14]([O:15][CH3:16])[cH:17][cH:18]1>>[CH3:1][CH2:2][CH2:3][CH2:4][n:5]1[cH:6][cH:7][c:8]2[cH:9][c:10](-[c:11]3[cH:12][cH:13][c:14]([O:15][CH3:16])[cH:17][cH:18]3)[cH:19][cH:20][c:21]12
CCCCn1ccc2cc(Br)ccc21.COc1ccc(B(O)O)cc1
CCCCn1ccc2cc(-c3ccc(OC)cc3)ccc21
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
42e21206f0250bb469664981cf521bd21ce6ff7bf8a8e9271f94397f7d3b79cb
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc3[nH]ccc3c2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](:[#7;a:5]):[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[#7;a:5]:[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]):[c:7]:[c:6]:1
null
[]
null
null
null
null
The title compound was prepared from 5-bromo-1-butyl-1H-indole (Step 1 of Example 29) and 4-methoxyphenylboronic acid in substantially the same manner, as described in Step 2 of Example 25. The product was obtained as an oil. Mass spectrum (ESI, [M+H]+) m/z 280.1 HNMR (400 MHz, DMSO-d6): δ 7.72 (s, 1H), 7.58 (dd, 2H, J...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1
HBr.B
null
null
null
CCCCn1ccc2cc(Br)ccc21.COc1ccc(B(O)O)cc1>>CCCCn1ccc2cc(-c3ccc(OC)cc3)ccc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-473ccea54dc34b72b66077d4b107335b
CCCCn1ccc2cc(Br)ccc21.OB(O)c1ccc(C(F)(F)F)cc1>>CCCCn1ccc2cc(-c3ccc(C(F)(F)F)cc3)ccc21
BrC=1C=C2C=CN(C2=CC1)CCCC.FC(C1=CC=C(C=C1)B(O)O)(F)F>>C(CCC)N1C=CC2=CC(=CC=C12)C1=CC=C(C=C1)C(F)(F)F
Br[c:10]1[cH:9][c:8]2[cH:7][cH:6][n:5]([CH2:4][CH2:3][CH2:2][CH3:1])[c:23]2[cH:22][cH:21]1.OB(O)[c:11]1[cH:12][cH:13][c:14]([C:15]([F:16])([F:17])[F:18])[cH:19][cH:20]1>>[CH3:1][CH2:2][CH2:3][CH2:4][n:5]1[cH:6][cH:7][c:8]2[cH:9][c:10](-[c:11]3[cH:12][cH:13][c:14]([C:15]([F:16])([F:17])[F:18])[cH:19][cH:20]3)[cH:21][cH:...
CCCCn1ccc2cc(Br)ccc21.OB(O)c1ccc(C(F)(F)F)cc1
CCCCn1ccc2cc(-c3ccc(C(F)(F)F)cc3)ccc21
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
42e21206f0250bb469664981cf521bd21ce6ff7bf8a8e9271f94397f7d3b79cb
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc3[nH]ccc3c2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](:[#7;a:5]):[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[#7;a:5]:[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]):[c:7]:[c:6]:1
null
[]
null
null
null
null
The title compound was prepared from 5-bromo-1-butyl-1H-indole (Step 1 of Example 29) and 4-trifluoromethylphenylboronic acid in substantially the same manner, as described in Step 2 of Example 25. The product was obtained as an oil, mp: 52-53° C. Mass spectrum (APCI, [M+H]+) m/z 318. 1HNMR (400 MHz, DMSO-d6): δ 7.91-7...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1
HBr.B
null
null
null
CCCCn1ccc2cc(Br)ccc21.OB(O)c1ccc(C(F)(F)F)cc1>>CCCCn1ccc2cc(-c3ccc(C(F)(F)F)cc3)ccc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-7315e87d178f4f0fa5176d9d518a0505
Brc1ccc2[nH]ccc2c1.CC(C)(C)c1ccc(CBr)cc1>>CC(C)(C)c1ccc(Cn2ccc3cc(Br)ccc32)cc1
C(C)(C)(C)C1=CC=C(CBr)C=C1.BrC=1C=C2C=CNC2=CC1>>BrC=1C=C2C=CN(C2=CC1)CC1=CC=C(C=C1)C(C)(C)C
[nH:10]1[cH:11][cH:12][c:13]2[cH:14][c:15]([Br:16])[cH:17][cH:18][c:19]12.Br[CH2:9][c:8]1[cH:7][cH:6][c:5]([C:2]([CH3:1])([CH3:3])[CH3:4])[cH:21][cH:20]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[c:5]1[cH:6][cH:7][c:8]([CH2:9][n:10]2[cH:11][cH:12][c:13]3[cH:14][c:15]([Br:16])[cH:17][cH:18][c:19]23)[cH:20][cH:21]1
Brc1ccc2[nH]ccc2c1.CC(C)(C)c1ccc(CBr)cc1
CC(C)(C)c1ccc(Cn2ccc3cc(Br)ccc32)cc1
null
null
null
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
92cc004fc3e2a92f5c9aa0385cdf93f1126e35d5aa485f4f5fe9240c9543c8fe
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ccc(Cn2ccc3ccccc32)cc1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[c:5]:[c:6]1:[c:7]:[c:8]:[c:9]:[nH;D2;+0:10]:1>>[c:5]:[c:6]1:[c:7]:[c:8]:[c:9]:[n;H0;D3;+0:10]:1-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
97
[{"value": 97.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The title compound was prepared from 4-(tert-butyl)benzyl bromide (180 g, 768 mmol) and 5-bromoindole (152 g, 768 mmol) in substantially the same manner, as described in Step 1 of Example 25. The product (257 g, 97%) was obtained as a yellow solid, mp: 108-109° C. Mass spectrum (ESI, [M+H]+) m/z 342. 1HNMR (400 MHz, DM...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
c1ccccc1.c1ccc2[nH]ccc2c1
HBr
null
null
null
Brc1ccc2[nH]ccc2c1.CC(C)(C)c1ccc(CBr)cc1>>CC(C)(C)c1ccc(Cn2ccc3cc(Br)ccc32)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f29b65b14c4c478ab1b106ae40f55161
CC(C)(C)c1ccc(Cn2ccc3cc(Br)ccc32)cc1.Cc1cccc(B(O)O)c1>>Cc1cccc(-c2ccc3c(ccn3Cc3ccc(C(C)(C)C)cc3)c2)c1
CC=1C=C(C=CC1)B(O)O.BrC=1C=C2C=CN(C2=CC1)CC1=CC=C(C=C1)C(C)(C)C.CC=1C=C(C=CC1)B(O)O.C([O-])([O-])=O.[K+].[K+].BrC=1C=C2C=CN(C2=CC1)CC1=CC=C(C=C1)C(C)(C)C>>C(C)(C)(C)C1=CC=C(CN2C=CC3=CC(=CC=C23)C2=CC(=CC=C2)C)C=C1
Br[c:7]1[cH:8][cH:9][c:10]2[c:11]([cH:12][cH:13][n:14]2[CH2:15][c:16]2[cH:17][cH:18][c:19]([C:20]([CH3:21])([CH3:22])[CH3:23])[cH:24][cH:25]2)[cH:26]1.OB(O)[c:6]1[cH:5][cH:4][cH:3][c:2]([CH3:1])[cH:27]1>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]3[c:11]([cH:12][cH:13][n:14]3[CH2:15][c:16]3[cH:17][cH...
CC(C)(C)c1ccc(Cn2ccc3cc(Br)ccc32)cc1.Cc1cccc(B(O)O)c1
Cc1cccc(-c2ccc3c(ccn3Cc3ccc(C(C)(C)C)cc3)c2)c1
null
[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC.C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-]
O1CCOCC1.O
C-C Coupling
Suzuki coupling with boronic acids
42e21206f0250bb469664981cf521bd21ce6ff7bf8a8e9271f94397f7d3b79cb
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](:[#7;a:5]):[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[#7;a:5]:[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]):[c:7]:[c:6]:1
73
[{"value": 73.0, "product": "C(C)(C)(C)C1=CC=C(CN2C=CC3=CC(=CC=C23)C2=CC(=CC=C2)C)C=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 72.9, "product": "C(C)(C)(C)C1=CC=C(CN2C=CC3=CC(=CC=C23)C2=CC(=CC=C2)C)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
70
CELSIUS
null
null
The mixture of 5-bromo-1-(4-tert-butylbenzyl)-1H-indole (67.5 g, 197.2 mmol), 3-methylbenzeneboronic acid (27.6 g, 197.2 mmol), potassium carbonate (27.2 g, 493 mmol), palladium(II) acetate (0.338 g) and tetrabutylammonium bromide (63.5 g, 197.2 mmol) in 10% dioxane in water (degassed, 1.72 L) was stirred at 70° C. The...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccccc1.c1ccc2[nH]ccc2c1
c1ccccc1.c1ccc2[nH]ccc2c1.c1ccccc1
HBr.B
[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC.C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].O1CCOCC1.O
70
null
CC(C)(C)c1ccc(Cn2ccc3cc(Br)ccc32)cc1.Cc1cccc(B(O)O)c1>[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC.C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].O1CCOCC1.O>Cc1cccc(-c2ccc3c(ccn3Cc3ccc(C(C)(C)C)cc3)c2)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-9374a454b9cc4db5977db909ad4c6745
CC(C)(C)c1ccc(Cn2ccc3cc(Br)ccc32)cc1.COc1cccc(B(O)O)c1>>COc1cccc(-c2ccc3c(ccn3Cc3ccc(C(C)(C)C)cc3)c2)c1
BrC=1C=C2C=CN(C2=CC1)CC1=CC=C(C=C1)C(C)(C)C.COC=1C=C(C=CC1)B(O)O>>C(C)(C)(C)C1=CC=C(CN2C=CC3=CC(=CC=C23)C2=CC(=CC=C2)OC)C=C1
Br[c:8]1[cH:9][cH:10][c:11]2[c:12]([cH:13][cH:14][n:15]2[CH2:16][c:17]2[cH:18][cH:19][c:20]([C:21]([CH3:22])([CH3:23])[CH3:24])[cH:25][cH:26]2)[cH:27]1.OB(O)[c:7]1[cH:6][cH:5][cH:4][c:3]([O:2][CH3:1])[cH:28]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][c:11]3[c:12]([cH:13][cH:14][n:15]3[CH2:16][c:17...
CC(C)(C)c1ccc(Cn2ccc3cc(Br)ccc32)cc1.COc1cccc(B(O)O)c1
COc1cccc(-c2ccc3c(ccn3Cc3ccc(C(C)(C)C)cc3)c2)c1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
42e21206f0250bb469664981cf521bd21ce6ff7bf8a8e9271f94397f7d3b79cb
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](:[#7;a:5]):[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[#7;a:5]:[c:4]1:[c:6]:[c:7]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]):[c:2]:[c:3]:1
null
[]
null
null
null
null
The title compound was prepared from 5-bromo-1-[4-(tert-butyl)benzyl]-1H-indole (Step 1 of Example 34) and 3-methoxyphenylboronic acid in substantially the same manner, as described in Step 2 of Example 25. The product was obtained as an oil. Mass spectrum (ESI, [M+H]+) m/z 370. 1HNMR (400 MHz, DMSO-d6): δ 7.81 (s, 1H)...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccccc1.c1ccc2[nH]ccc2c1
c1ccccc1.c1ccc2[nH]ccc2c1.c1ccccc1
HBr.B
null
null
null
CC(C)(C)c1ccc(Cn2ccc3cc(Br)ccc32)cc1.COc1cccc(B(O)O)c1>>COc1cccc(-c2ccc3c(ccn3Cc3ccc(C(C)(C)C)cc3)c2)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-33fce8c9c52d453897e4300df2d0ba90
CC(C)(C)c1ccc(B(O)O)cc1.CC(C)(C)c1ccc(Cn2ccc3cc(Br)ccc32)cc1>>CC(C)(C)c1ccc(Cn2ccc3cc(-c4ccc(C(C)(C)C)cc4)ccc32)cc1
BrC=1C=C2C=CN(C2=CC1)CC1=CC=C(C=C1)C(C)(C)C.C(C)(C)(C)C1=CC=C(C=C1)B(O)O>>C(C)(C)(C)C1=CC=C(CN2C=CC3=CC(=CC=C23)C2=CC=C(C=C2)C(C)(C)C)C=C1
OB(O)[c:16]1[cH:17][cH:18][c:19]([C:20]([CH3:21])([CH3:22])[CH3:23])[cH:24][cH:25]1.Br[c:15]1[cH:14][c:13]2[cH:12][cH:11][n:10]([CH2:9][c:8]3[cH:7][cH:6][c:5]([C:2]([CH3:1])([CH3:3])[CH3:4])[cH:30][cH:29]3)[c:28]2[cH:27][cH:26]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[c:5]1[cH:6][cH:7][c:8]([CH2:9][n:10]2[cH:11][cH:12][c:13]3[...
CC(C)(C)c1ccc(B(O)O)cc1.CC(C)(C)c1ccc(Cn2ccc3cc(Br)ccc32)cc1
CC(C)(C)c1ccc(Cn2ccc3cc(-c4ccc(C(C)(C)C)cc4)ccc32)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
42e21206f0250bb469664981cf521bd21ce6ff7bf8a8e9271f94397f7d3b79cb
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](:[#7;a:5]):[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[#7;a:5]:[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]):[c:7]:[c:6]:1
null
[]
null
null
null
null
The title compound was prepared from 5-bromo-1-[4-(tert-butyl)benzyl]-1H-indole (Step 1 of Example 34) and 4-(tert-butyl)phenylboronic acid in substantially the same manner, as described in Step 2 of Example 25. The product was obtained as an off-white solid, mp: 167-168° C. Mass spectrum (ESI, [M+H]+) m/z 396. 1 HNMR ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccccc1.c1ccc2[nH]ccc2c1.c1ccccc1
HBr.B
null
null
null
CC(C)(C)c1ccc(B(O)O)cc1.CC(C)(C)c1ccc(Cn2ccc3cc(Br)ccc32)cc1>>CC(C)(C)c1ccc(Cn2ccc3cc(-c4ccc(C(C)(C)C)cc4)ccc32)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-10349e0697f84ed19a2fddcc69306e49
CC(C)(C)c1ccc(Cn2ccc3cc(Br)ccc32)cc1.OB(O)c1cccc(Cl)c1>>CC(C)(C)c1ccc(Cn2ccc3cc(-c4cccc(Cl)c4)ccc32)cc1
BrC=1C=C2C=CN(C2=CC1)CC1=CC=C(C=C1)C(C)(C)C.ClC=1C=C(C=CC1)B(O)O>>C(C)(C)(C)C1=CC=C(CN2C=CC3=CC(=CC=C23)C2=CC(=CC=C2)Cl)C=C1
Br[c:15]1[cH:14][c:13]2[cH:12][cH:11][n:10]([CH2:9][c:8]3[cH:7][cH:6][c:5]([C:2]([CH3:1])([CH3:3])[CH3:4])[cH:27][cH:26]3)[c:25]2[cH:24][cH:23]1.OB(O)[c:16]1[cH:17][cH:18][cH:19][c:20]([Cl:21])[cH:22]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[c:5]1[cH:6][cH:7][c:8]([CH2:9][n:10]2[cH:11][cH:12][c:13]3[cH:14][c:15](-[c:16]4[cH:17...
CC(C)(C)c1ccc(Cn2ccc3cc(Br)ccc32)cc1.OB(O)c1cccc(Cl)c1
CC(C)(C)c1ccc(Cn2ccc3cc(-c4cccc(Cl)c4)ccc32)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
42e21206f0250bb469664981cf521bd21ce6ff7bf8a8e9271f94397f7d3b79cb
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](:[#7;a:5]):[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[#7;a:5]:[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]):[c:7]:[c:6]:1
null
[]
null
null
null
null
The title compound was prepared from 5-bromo-1-[4-(tert-butyl)benzyl]-1H-indole (Step 1 of Example 34) and 3-chlorophenylboronic acid in substantially the same manner, as described in Step 2 of Example 25. The product was obtained as an oil. Mass spectrum (ESI, [M+H]+) m/z 374. 1HNMR (400 MHz, DMSO-d6): δ 7.86 (d, 1H, ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccccc1.c1ccc2[nH]ccc2c1.c1ccccc1
HBr.B
null
null
null
CC(C)(C)c1ccc(Cn2ccc3cc(Br)ccc32)cc1.OB(O)c1cccc(Cl)c1>>CC(C)(C)c1ccc(Cn2ccc3cc(-c4cccc(Cl)c4)ccc32)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d0c5fe00562440babe963c5778202b21
CC(C)(C)c1ccc(Cn2ccc3cc(Br)ccc32)cc1.OB(O)c1ccc(Cl)cc1>>CC(C)(C)c1ccc(Cn2ccc3cc(-c4ccc(Cl)cc4)ccc32)cc1
BrC=1C=C2C=CN(C2=CC1)CC1=CC=C(C=C1)C(C)(C)C.ClC1=CC=C(C=C1)B(O)O>>C(C)(C)(C)C1=CC=C(CN2C=CC3=CC(=CC=C23)C2=CC=C(C=C2)Cl)C=C1
Br[c:15]1[cH:14][c:13]2[cH:12][cH:11][n:10]([CH2:9][c:8]3[cH:7][cH:6][c:5]([C:2]([CH3:1])([CH3:3])[CH3:4])[cH:27][cH:26]3)[c:25]2[cH:24][cH:23]1.OB(O)[c:16]1[cH:17][cH:18][c:19]([Cl:20])[cH:21][cH:22]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[c:5]1[cH:6][cH:7][c:8]([CH2:9][n:10]2[cH:11][cH:12][c:13]3[cH:14][c:15](-[c:16]4[cH:17...
CC(C)(C)c1ccc(Cn2ccc3cc(Br)ccc32)cc1.OB(O)c1ccc(Cl)cc1
CC(C)(C)c1ccc(Cn2ccc3cc(-c4ccc(Cl)cc4)ccc32)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
42e21206f0250bb469664981cf521bd21ce6ff7bf8a8e9271f94397f7d3b79cb
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](:[#7;a:5]):[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[#7;a:5]:[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]):[c:7]:[c:6]:1
null
[]
null
null
null
null
The title compound was prepared from 5-bromo-1-[4-(tert-butyl)benzyl]-1H-indole (Step 1 of Example 34) and 4-chlorophenylboronic acid in substantially the same manner, as described in Step 2 of Example 25. The product was obtained as an oil. Mass spectrum (ESI, [M+H]+) m/z 374. 1HNMR (400 MHz, DMSO-d6): δ 7.82 (d, 1H, ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccccc1.c1ccc2[nH]ccc2c1.c1ccccc1
HBr.B
null
null
null
CC(C)(C)c1ccc(Cn2ccc3cc(Br)ccc32)cc1.OB(O)c1ccc(Cl)cc1>>CC(C)(C)c1ccc(Cn2ccc3cc(-c4ccc(Cl)cc4)ccc32)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-341dbc47d56e4f5d976add51f58dcf27
CC(C)(C)c1ccc(Cn2ccc3cc(Br)ccc32)cc1.Cc1ccccc1B(O)O>>Cc1ccccc1-c1ccc2c(ccn2Cc2ccc(C(C)(C)C)cc2)c1
BrC=1C=C2C=CN(C2=CC1)CC1=CC=C(C=C1)C(C)(C)C.CC1=C(C=CC=C1)B(O)O>>C(C)(C)(C)C1=CC=C(CN2C=CC3=CC(=CC=C23)C2=C(C=CC=C2)C)C=C1
Br[c:8]1[cH:9][cH:10][c:11]2[c:12]([cH:13][cH:14][n:15]2[CH2:16][c:17]2[cH:18][cH:19][c:20]([C:21]([CH3:22])([CH3:23])[CH3:24])[cH:25][cH:26]2)[cH:27]1.OB(O)[c:7]1[c:2]([CH3:1])[cH:3][cH:4][cH:5][cH:6]1>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1-[c:8]1[cH:9][cH:10][c:11]2[c:12]([cH:13][cH:14][n:15]2[CH2:16][c:17]2[cH...
CC(C)(C)c1ccc(Cn2ccc3cc(Br)ccc32)cc1.Cc1ccccc1B(O)O
Cc1ccccc1-c1ccc2c(ccn2Cc2ccc(C(C)(C)C)cc2)c1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
42e21206f0250bb469664981cf521bd21ce6ff7bf8a8e9271f94397f7d3b79cb
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](:[#7;a:5]):[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11](-[C;D1;H3:12]):[c:13]>>[#7;a:5]:[c:4]1:[c:6]:[c:7]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11](-[C;D1;H3:12]):[c:13]):[c:2]:[c:3]:1
null
[]
null
null
null
null
The title compound was prepared from 5-bromo-1-[4-(tert-butyl)benzyl]-1H-indole (Step 1 of Example 34) and 2-methylphenylboronic acid in substantially the same manner, as described in Step 2 of Example 25. The product was obtained as a brown oil. Mass spectrum (ESI, [M+H]+) m/z 354. 1HNMR (400 MHz, DMSO-d6): δ 7.53 (d,...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccccc1.c1ccc2[nH]ccc2c1
c1ccccc1.c1ccc2[nH]ccc2c1.c1ccccc1
HBr.B
null
null
null
CC(C)(C)c1ccc(Cn2ccc3cc(Br)ccc32)cc1.Cc1ccccc1B(O)O>>Cc1ccccc1-c1ccc2c(ccn2Cc2ccc(C(C)(C)C)cc2)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-8510fa620e884ee7af4c9cee7d7feab0
Brc1ccc2[nH]ccc2c1.CCC(CC)CBr>>CCC(CC)Cn1ccc2cc(Br)ccc21
BrCC(CC)CC.BrC=1C=C2C=CNC2=CC1>>BrC=1C=C2C=CN(C2=CC1)CC(CC)CC
[nH:7]1[cH:8][cH:9][c:10]2[cH:11][c:12]([Br:13])[cH:14][cH:15][c:16]12.Br[CH2:6][CH:3]([CH2:2][CH3:1])[CH2:4][CH3:5]>>[CH3:1][CH2:2][CH:3]([CH2:4][CH3:5])[CH2:6][n:7]1[cH:8][cH:9][c:10]2[cH:11][c:12]([Br:13])[cH:14][cH:15][c:16]12
Brc1ccc2[nH]ccc2c1.CCC(CC)CBr
CCC(CC)Cn1ccc2cc(Br)ccc21
null
null
null
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
92cc004fc3e2a92f5c9aa0385cdf93f1126e35d5aa485f4f5fe9240c9543c8fe
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ccc2[nH]ccc2c1
Br-[CH2;D2;+0:1]-[C:2](-[C:3])-[C:4].[c:5]:[c:6]1:[c:7]:[c:8]:[c:9]:[nH;D2;+0:10]:1>>[C:3]-[C:2](-[C:4])-[CH2;D2;+0:1]-[n;H0;D3;+0:10]1:[c:9]:[c:8]:[c:7]:[c:6]:1:[c:5]
62
[{"value": 62.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The title compound was prepared from 1-bromo-2-ethylbutane (14.14 mL, 101 mmol) and 5-bromoindole (20 g, 101 mmol) in substantially the same manner, as described in Step 1 of Example 25. The product (17.78 g, 62%) was obtained as a colorless oil. Mass spectrum (ESI, [M+H]+) m/z 280. 1 HNMR (400 MHz, DMSO-d6): δ 7.71 (d...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
HBr
null
null
null
Brc1ccc2[nH]ccc2c1.CCC(CC)CBr>>CCC(CC)Cn1ccc2cc(Br)ccc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b2bd910bae3f4c60a9cb3f3c9838f554
CCC(CC)Cn1ccc2cc(Br)ccc21.OB(O)c1ccc(OC(F)(F)F)cc1>>CCC(CC)Cn1ccc2cc(-c3ccc(OC(F)(F)F)cc3)ccc21
BrC=1C=C2C=CN(C2=CC1)CC(CC)CC.FC(OC1=CC=C(C=C1)B(O)O)(F)F>>C(C)C(CN1C=CC2=CC(=CC=C12)C1=CC=C(C=C1)OC(F)(F)F)CC
Br[c:12]1[cH:11][c:10]2[cH:9][cH:8][n:7]([CH2:6][CH:3]([CH2:2][CH3:1])[CH2:4][CH3:5])[c:26]2[cH:25][cH:24]1.OB(O)[c:13]1[cH:14][cH:15][c:16]([O:17][C:18]([F:19])([F:20])[F:21])[cH:22][cH:23]1>>[CH3:1][CH2:2][CH:3]([CH2:4][CH3:5])[CH2:6][n:7]1[cH:8][cH:9][c:10]2[cH:11][c:12](-[c:13]3[cH:14][cH:15][c:16]([O:17][C:18]([F:...
CCC(CC)Cn1ccc2cc(Br)ccc21.OB(O)c1ccc(OC(F)(F)F)cc1
CCC(CC)Cn1ccc2cc(-c3ccc(OC(F)(F)F)cc3)ccc21
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
42e21206f0250bb469664981cf521bd21ce6ff7bf8a8e9271f94397f7d3b79cb
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc3[nH]ccc3c2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](:[#7;a:5]):[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[#7;a:5]:[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]):[c:7]:[c:6]:1
null
[]
null
null
null
null
The title compound was prepared from 5-bromo-1-(2-ethylbutyl)-1H-indole and 4-(trifluoromethoxy)phenylboronic acid in substantially the same manner, as described in Step 2 of Example 25. The product was obtained as an oil. Mass spectrum (APCI, [M+H]+) m/z 362. 1HNMR (300 MHz, DMSO-d6): δ 7.82 (s, 1H), 7.77 (d, 2H, J=8....
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1
HBr.B
null
null
null
CCC(CC)Cn1ccc2cc(Br)ccc21.OB(O)c1ccc(OC(F)(F)F)cc1>>CCC(CC)Cn1ccc2cc(-c3ccc(OC(F)(F)F)cc3)ccc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d773cb8dbbcf421e89bf4e4e2f23ad48
CCOC(=O)c1cc2cc(Br)ccc2[nH]1.Cc1ccc(CBr)cc1>>CCOC(=O)c1cc2cc(Br)ccc2n1Cc1ccc(C)cc1
BrC=1C=C2C=C(NC2=CC1)C(=O)OCC.CC1=CC=C(CBr)C=C1.CN(C)C=O>>BrC=1C=C2C=C(N(C2=CC1)CC1=CC=C(C=C1)C)C(=O)OCC
[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][c:8]2[cH:9][c:10]([Br:11])[cH:12][cH:13][c:14]2[nH:15]1.Br[CH2:16][c:17]1[cH:18][cH:19][c:20]([CH3:21])[cH:22][cH:23]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][c:8]2[cH:9][c:10]([Br:11])[cH:12][cH:13][c:14]2[n:15]1[CH2:16][c:17]1[cH:18][cH:19][c:20]([CH3:21])[cH:22][cH:...
CCOC(=O)c1cc2cc(Br)ccc2[nH]1.Cc1ccc(CBr)cc1
CCOC(=O)c1cc2cc(Br)ccc2n1Cc1ccc(C)cc1
null
null
null
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
92cc004fc3e2a92f5c9aa0385cdf93f1126e35d5aa485f4f5fe9240c9543c8fe
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ccc(Cn2ccc3ccccc32)cc1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[C:5]-[#8:6]-[C:7](=[O;D1;H0:8])-[c:9]1:[c:10]:[c:11]:[c:12](:[c:13]):[nH;D2;+0:14]:1>>[C:5]-[#8:6]-[C:7](=[O;D1;H0:8])-[c:9]1:[c:10]:[c:11]:[c:12](:[c:13]):[n;H0;D3;+0:14]:1-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
The title compound was prepared from ethyl 5-bromo-1H-indole-2-carboxylate and 4-methylbenzyl bromide in substantially the same manner, as described in Step 1 of Example 25. The product was obtained as a semi-solid contained 0.8 mole equivalent DMF. Mass spectrum (ESI, [M+H]+) m/z 372. 1H NMR (400 MHz, DMSO-d6) δ 7.93 ...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.c1ccccc1
HBr
null
null
null
CCOC(=O)c1cc2cc(Br)ccc2[nH]1.Cc1ccc(CBr)cc1>>CCOC(=O)c1cc2cc(Br)ccc2n1Cc1ccc(C)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a4be1e5594f1414f8eb7b885536308c5
CCOC(=O)c1cc2cc(Br)ccc2n1Cc1ccc(C)cc1.OB(O)c1ccc(OC(F)(F)F)cc1>>CCOC(=O)c1cc2cc(-c3ccc(OC(F)(F)F)cc3)ccc2n1Cc1ccc(C)cc1
BrC=1C=C2C=C(N(C2=CC1)CC1=CC=C(C=C1)C)C(=O)OCC.FC(OC1=CC=C(C=C1)B(O)O)(F)F>>CC1=CC=C(CN2C(=CC3=CC(=CC=C23)C2=CC=C(C=C2)OC(F)(F)F)C(=O)OCC)C=C1
Br[c:10]1[cH:9][c:8]2[cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[n:25]([CH2:26][c:27]3[cH:28][cH:29][c:30]([CH3:31])[cH:32][cH:33]3)[c:24]2[cH:23][cH:22]1.OB(O)[c:11]1[cH:12][cH:13][c:14]([O:15][C:16]([F:17])([F:18])[F:19])[cH:20][cH:21]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][c:8]2[cH:9][c:10](-[c:11]3[cH:12]...
CCOC(=O)c1cc2cc(Br)ccc2n1Cc1ccc(C)cc1.OB(O)c1ccc(OC(F)(F)F)cc1
CCOC(=O)c1cc2cc(-c3ccc(OC(F)(F)F)cc3)ccc2n1Cc1ccc(C)cc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
42e21206f0250bb469664981cf521bd21ce6ff7bf8a8e9271f94397f7d3b79cb
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](:[#7;a:5]):[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[#7;a:5]:[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]):[c:7]:[c:6]:1
null
[]
null
null
null
null
The title compound was prepared from ethyl 5-bromo-1-(4-methylbenzyl)-1H-indole-2-carboxylate and 4-(trifluoromethoxy)phenylboronic acid in substantially the same manner, as described in Step 2 of Example 25. The product was obtained as an off-white solid, m.p. 77-78° C. Mass spectrum (ESI, [M+H]+) m/z 454. 1H NMR (400...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1.c1ccccc1
HBr.B
null
null
null
CCOC(=O)c1cc2cc(Br)ccc2n1Cc1ccc(C)cc1.OB(O)c1ccc(OC(F)(F)F)cc1>>CCOC(=O)c1cc2cc(-c3ccc(OC(F)(F)F)cc3)ccc2n1Cc1ccc(C)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-71d391290e9f492c834108966b3a84d2
CCOC(=O)c1cc2cc(-c3ccc(OC(F)(F)F)cc3)ccc2n1Cc1ccc(C)cc1>>Cc1ccc(Cn2c(CO)cc3cc(-c4ccc(OC(F)(F)F)cc4)ccc32)cc1
[H-].[Al+3].[Li+].[H-].[H-].[H-].CC1=CC=C(CN2C(=CC3=CC(=CC=C23)C2=CC=C(C=C2)OC(F)(F)F)C(=O)OCC)C=C1>>CC1=CC=C(CN2C(=CC3=CC(=CC=C23)C2=CC=C(C=C2)OC(F)(F)F)CO)C=C1
CCO[C:9]([c:8]1[n:7]([CH2:6][c:5]2[cH:4][cH:3][c:2]([CH3:1])[cH:30][cH:29]2)[c:28]2[c:12]([cH:11]1)[cH:13][c:14](-[c:15]1[cH:16][cH:17][c:18]([O:19][C:20]([F:21])([F:22])[F:23])[cH:24][cH:25]1)[cH:26][cH:27]2)=[O:10]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([CH2:6][n:7]2[c:8]([CH2:9][OH:10])[cH:11][c:12]3[cH:13][c:14](-[c:15]4[...
CCOC(=O)c1cc2cc(-c3ccc(OC(F)(F)F)cc3)ccc2n1Cc1ccc(C)cc1
Cc1ccc(Cn2c(CO)cc3cc(-c4ccc(OC(F)(F)F)cc4)ccc32)cc1
null
null
C(C)OCC
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
C-C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3](:[c:4]):[#7;a:5](-[C:6]):[c:7]>>[C:6]-[#7;a:5](:[c:7]):[c:3](-[CH2;D2;+0:1]-[OH;D1;+0:2]):[c:4]
86.2
[{"value": 86.0, "product": "CC1=CC=C(CN2C(=CC3=CC(=CC=C23)C2=CC=C(C=C2)OC(F)(F)F)CO)C=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 86.2, "product": "CC1=CC=C(CN2C(=CC3=CC(=CC=C23)C2=CC=C(C=C2)OC(F)(F)F)CO)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
5
HOUR
Lithium aluminum hydride (0.244 g, 6.1 mmol) was added portionwise to a stirring solution of ethyl 1-(4-methylbenzyl)-5-[4-(trifluoromethoxy)phenyl]-1H-indole-2-carboxylate (2.0 g, 4.4 mmol) in ethyl ether (17 mL) at 0° C. under a nitrogen atmosphere over a period of 5 minutes. The mixture was then warmed up to room te...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
c1ccccc1.c1ccc2[nH]ccc2c1.c1ccccc1
HO-
C(C)OCC
null
5
CCOC(=O)c1cc2cc(-c3ccc(OC(F)(F)F)cc3)ccc2n1Cc1ccc(C)cc1>C(C)OCC>Cc1ccc(Cn2c(CO)cc3cc(-c4ccc(OC(F)(F)F)cc4)ccc32)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-80d80c1c55fb4578bdb49d8fb3a9d1a5
CC(=O)Cl.Cc1ccc(Cn2c(CO)cc3cc(-c4ccc(OC(F)(F)F)cc4)ccc32)cc1>>CC(=O)OCc1cc2cc(-c3ccc(OC(F)(F)F)cc3)ccc2n1Cc1ccc(C)cc1
C(C)(=O)Cl.CC1=CC=C(CN2C(=CC3=CC(=CC=C23)C2=CC=C(C=C2)OC(F)(F)F)CO)C=C1.C(C)(C)N(C(C)C)CC>>C(C)(=O)OCC=1N(C2=CC=C(C=C2C1)C1=CC=C(C=C1)OC(F)(F)F)CC1=CC=C(C=C1)C
Cl[C:2]([CH3:1])=[O:3].[OH:4][CH2:5][c:6]1[cH:7][c:8]2[cH:9][c:10](-[c:11]3[cH:12][cH:13][c:14]([O:15][C:16]([F:17])([F:18])[F:19])[cH:20][cH:21]3)[cH:22][cH:23][c:24]2[n:25]1[CH2:26][c:27]1[cH:28][cH:29][c:30]([CH3:31])[cH:32][cH:33]1>>[CH3:1][C:2](=[O:3])[O:4][CH2:5][c:6]1[cH:7][c:8]2[cH:9][c:10](-[c:11]3[cH:12][cH:1...
CC(=O)Cl.Cc1ccc(Cn2c(CO)cc3cc(-c4ccc(OC(F)(F)F)cc4)ccc32)cc1
CC(=O)OCc1cc2cc(-c3ccc(OC(F)(F)F)cc3)ccc2n1Cc1ccc(C)cc1
null
null
C(Cl)Cl
Acylation
Schotten-Baumann to ester
6cefe709828c5bd4655f254e75d5dff9e8876e192e7dd47256c1bc0067bc5291
d8a7643b81ed07a6f633aa99465180dfa0565e61ae25aef36338ebb9837c9cef
c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
Cl-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[#7;a:4]:[c:5]-[C:6]-[OH;D1;+0:7]>>[#7;a:4]:[c:5]-[C:6]-[O;H0;D2;+0:7]-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3]
99.9
[{"value": 99.6, "product": "C(C)(=O)OCC=1N(C2=CC=C(C=C2C1)C1=CC=C(C=C1)OC(F)(F)F)CC1=CC=C(C=C1)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 99.9, "product": "C(C)(=O)OCC=1N(C2=CC=C(C=C2C1)C1=CC=C(C=C1)OC(F)(F)F)CC1=CC=C(C=C1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
Acetyl chloride (0.222 mL, 3.08 mmol) was added to a stirring solution of {1-(4-methylbenzyl)-5-[4-(trifluoromethoxy)phenyl]-1H-indol-2-yl}methanol (0.507 g, 1.23 mmol) and N,N-diisopropylethylamine (0.547 mL, 3.08 mmol) in methylene chloride (8 mL) at 0° C. under a nitrogen atmosphere over a period of 5 minutes. After...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary alcohol
Ester
null
null
c1ccc2[nH]ccc2c1.c1ccccc1.c1ccccc1
HCl
C(Cl)Cl
null
8
CC(=O)Cl.Cc1ccc(Cn2c(CO)cc3cc(-c4ccc(OC(F)(F)F)cc4)ccc32)cc1>C(Cl)Cl>CC(=O)OCc1cc2cc(-c3ccc(OC(F)(F)F)cc3)ccc2n1Cc1ccc(C)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e835db01a31448aca69cfb8e455ba8aa
BrCc1ccccc1.CCOC(=O)c1cc2cc(Br)ccc2[nH]1>>CCOC(=O)c1cc2cc(Br)ccc2n1Cc1ccccc1
BrC=1C=C2C=C(NC2=CC1)C(=O)OCC.C(C1=CC=CC=C1)Br>>BrC=1C=C2C=C(N(C2=CC1)CC1=CC=CC=C1)C(=O)OCC
Br[CH2:16][c:17]1[cH:18][cH:19][cH:20][cH:21][cH:22]1.[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][c:8]2[cH:9][c:10]([Br:11])[cH:12][cH:13][c:14]2[nH:15]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][c:8]2[cH:9][c:10]([Br:11])[cH:12][cH:13][c:14]2[n:15]1[CH2:16][c:17]1[cH:18][cH:19][cH:20][cH:21][cH:22]1
BrCc1ccccc1.CCOC(=O)c1cc2cc(Br)ccc2[nH]1
CCOC(=O)c1cc2cc(Br)ccc2n1Cc1ccccc1
null
null
null
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
92cc004fc3e2a92f5c9aa0385cdf93f1126e35d5aa485f4f5fe9240c9543c8fe
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
c1ccc(Cn2ccc3ccccc32)cc1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[C:5]-[#8:6]-[C:7](=[O;D1;H0:8])-[c:9]1:[c:10]:[c:11]:[c:12](:[c:13]):[nH;D2;+0:14]:1>>[C:5]-[#8:6]-[C:7](=[O;D1;H0:8])-[c:9]1:[c:10]:[c:11]:[c:12](:[c:13]):[n;H0;D3;+0:14]:1-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
The title compound was prepared from ethyl 5-bromo-1H-indole-2-carboxylate and benzyl bromide in substantially the same manner, as described in Step 1 of Example 25. The product was obtained as a light yellow solid. Mass spectrum (ESI, [M+H]+) m/z 358.1 HNMR (300 MHz, DMSO-d6): δ 7.94 (s, 1H), 7.55 (d, 1H, J=9.01 Hz), ...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.c1ccccc1
HBr
null
null
null
BrCc1ccccc1.CCOC(=O)c1cc2cc(Br)ccc2[nH]1>>CCOC(=O)c1cc2cc(Br)ccc2n1Cc1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5495bbecea264db89a9b958f4af142e1
CCOC(=O)c1cc2cc(Br)ccc2n1Cc1ccccc1.OB(O)c1ccc(OC(F)(F)F)cc1>>CCOC(=O)c1cc2cc(-c3ccc(OC(F)(F)F)cc3)ccc2n1Cc1ccccc1
BrC=1C=C2C=C(N(C2=CC1)CC1=CC=CC=C1)C(=O)OCC.FC(OC1=CC=C(C=C1)B(O)O)(F)F>>C(C1=CC=CC=C1)N1C(=CC2=CC(=CC=C12)C1=CC=C(C=C1)OC(F)(F)F)C(=O)OCC
Br[c:10]1[cH:9][c:8]2[cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[n:25]([CH2:26][c:27]3[cH:28][cH:29][cH:30][cH:31][cH:32]3)[c:24]2[cH:23][cH:22]1.OB(O)[c:11]1[cH:12][cH:13][c:14]([O:15][C:16]([F:17])([F:18])[F:19])[cH:20][cH:21]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][c:8]2[cH:9][c:10](-[c:11]3[cH:12][cH:13][c...
CCOC(=O)c1cc2cc(Br)ccc2n1Cc1ccccc1.OB(O)c1ccc(OC(F)(F)F)cc1
CCOC(=O)c1cc2cc(-c3ccc(OC(F)(F)F)cc3)ccc2n1Cc1ccccc1
null
null
null
C-C Coupling
Suzuki coupling with boronic acids
42e21206f0250bb469664981cf521bd21ce6ff7bf8a8e9271f94397f7d3b79cb
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](:[#7;a:5]):[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[#7;a:5]:[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]):[c:7]:[c:6]:1
null
[]
null
null
null
null
The title compound was prepared from ethyl 5-bromo-1-benzyl-1H-indole-2-carboxylate and 4-(trifluoromethoxy)phenylboronic acid in substantially the same manner, as described in Step 2 of Example 25. The product was obtained as an oil. Mass spectrum (ESI, [M+H]+) m/z 440. 1HNMR (400 MHz, DMSO-d6): δ 8.01 (s, 1H), 7.79 (...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1.c1ccccc1.c1ccccc1
HBr.B
null
null
null
CCOC(=O)c1cc2cc(Br)ccc2n1Cc1ccccc1.OB(O)c1ccc(OC(F)(F)F)cc1>>CCOC(=O)c1cc2cc(-c3ccc(OC(F)(F)F)cc3)ccc2n1Cc1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-94f437dd366c48669ce5e425d84773b9
CCOC(=O)c1cc2cc(-c3ccc(OC(F)(F)F)cc3)ccc2n1Cc1ccccc1>>OCc1cc2cc(-c3ccc(OC(F)(F)F)cc3)ccc2n1Cc1ccccc1
C(C1=CC=CC=C1)N1C(=CC2=CC(=CC=C12)C1=CC=C(C=C1)OC(F)(F)F)C(=O)OCC.[H-].[Al+3].[Li+].[H-].[H-].[H-]>>C(C1=CC=CC=C1)N1C(=CC2=CC(=CC=C12)C1=CC=C(C=C1)OC(F)(F)F)CO
CCO[C:2](=[O:1])[c:3]1[cH:4][c:5]2[cH:6][c:7](-[c:8]3[cH:9][cH:10][c:11]([O:12][C:13]([F:14])([F:15])[F:16])[cH:17][cH:18]3)[cH:19][cH:20][c:21]2[n:22]1[CH2:23][c:24]1[cH:25][cH:26][cH:27][cH:28][cH:29]1>>[OH:1][CH2:2][c:3]1[cH:4][c:5]2[cH:6][c:7](-[c:8]3[cH:9][cH:10][c:11]([O:12][C:13]([F:14])([F:15])[F:16])[cH:17][cH...
CCOC(=O)c1cc2cc(-c3ccc(OC(F)(F)F)cc3)ccc2n1Cc1ccccc1
OCc1cc2cc(-c3ccc(OC(F)(F)F)cc3)ccc2n1Cc1ccccc1
null
null
null
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
C-C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3](:[c:4]):[#7;a:5](-[C:6]):[c:7]>>[C:6]-[#7;a:5](:[c:7]):[c:3](-[CH2;D2;+0:1]-[OH;D1;+0:2]):[c:4]
null
[]
null
null
null
null
The title compound was prepared from Ethyl 1-benzyl-5-[4-(trifluoromethoxy)phenyl]-1H-indole-2-carboxylate (Step 2 of Example 25) and lithium aluminum hydride in substantially the same manner, as described in Step 1 of Example 21. The product was obtained as a white solid, mp: 108-109° C. Mass spectrum (ESI, [M+H]+) m/...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
c1ccc2[nH]ccc2c1.c1ccccc1.c1ccccc1
HO-
null
null
null
CCOC(=O)c1cc2cc(-c3ccc(OC(F)(F)F)cc3)ccc2n1Cc1ccccc1>>OCc1cc2cc(-c3ccc(OC(F)(F)F)cc3)ccc2n1Cc1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-7510a371f1a04711bd90311ce57847a5
Brc1ccc2[nH]ccc2c1.OB(O)c1cccc(Cl)c1>>Clc1cccc(-c2ccc3[nH]ccc3c2)c1
C(=O)([O-])[O-].[Na+].[Na+].BrC=1C=C2C=CNC2=CC1.ClC=1C=C(C=CC1)B(O)O.CCO.O>>ClC=1C=C(C=CC1)C=1C=C2C=CNC2=CC1
Br[c:7]1[cH:8][cH:9][c:10]2[nH:11][cH:12][cH:13][c:14]2[cH:15]1.OB(O)[c:6]1[cH:5][cH:4][cH:3][c:2]([Cl:1])[cH:16]1>>[Cl:1][c:2]1[cH:3][cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]3[nH:11][cH:12][cH:13][c:14]3[cH:15]2)[cH:16]1
Brc1ccc2[nH]ccc2c1.OB(O)c1cccc(Cl)c1
Clc1cccc(-c2ccc3[nH]ccc3c2)c1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O
C-C Coupling
Suzuki coupling with boronic acids
42e21206f0250bb469664981cf521bd21ce6ff7bf8a8e9271f94397f7d3b79cb
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
c1ccc(-c2ccc3[nH]ccc3c2)cc1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4](:[#7;a:5]):[c:6]:[c:7]:1.O-B(-O)-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]>>[#7;a:5]:[c:4]1:[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:8](:[c:9]:[c:10]):[c:11]:[c:12]):[c:7]:[c:6]:1
100.5
[{"value": 100.5, "product": "ClC=1C=C(C=CC1)C=1C=C2C=CNC2=CC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A stirred slurry of 4.23 g (40 mmol) Na2CO3, 1.84 g (9.4 mmol) 5-bromoindole, 1.88 g (10 mmol) 3-chlorophenylboronic acid, and 0.29 g (0.25 mmol) Pd(PPh3)4 in 50 mL 1:1 EtOH-water was heated to reflux for 2.5 hours. The reaction mixture was allowed to cool and was then poured into 400 mL water and extracted with EtOAc....
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccccc1.c1ccc2[nH]ccc2c1
c1ccccc1.c1ccc2[nH]ccc2c1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O
null
null
Brc1ccc2[nH]ccc2c1.OB(O)c1cccc(Cl)c1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O>Clc1cccc(-c2ccc3[nH]ccc3c2)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-947dac7a446e4ebf97672fc1bae21095
Clc1cccc(-c2ccc3[nH]ccc3c2)c1.O=S(=O)(Cl)c1ccccc1>>O=S(=O)(c1ccccc1)n1ccc2cc(-c3cccc(Cl)c3)ccc21
O.C1(=CC=CC=C1)S(=O)(=O)Cl.[H-].[Na+].ClC=1C=C(C=CC1)C=1C=C2C=CNC2=CC1>>C1(=CC=CC=C1)S(=O)(=O)N1C=CC2=CC(=CC=C12)C1=CC(=CC=C1)Cl
[nH:10]1[cH:11][cH:12][c:13]2[cH:14][c:15](-[c:16]3[cH:17][cH:18][cH:19][c:20]([Cl:21])[cH:22]3)[cH:23][cH:24][c:25]12.Cl[S:2](=[O:1])(=[O:3])[c:4]1[cH:5][cH:6][cH:7][cH:8][cH:9]1>>[O:1]=[S:2](=[O:3])([c:4]1[cH:5][cH:6][cH:7][cH:8][cH:9]1)[n:10]1[cH:11][cH:12][c:13]2[cH:14][c:15](-[c:16]3[cH:17][cH:18][cH:19][c:20]([Cl...
Clc1cccc(-c2ccc3[nH]ccc3c2)c1.O=S(=O)(Cl)c1ccccc1
O=S(=O)(c1ccccc1)n1ccc2cc(-c3cccc(Cl)c3)ccc21
null
null
C1CCOC1
Miscellaneous
OtherReaction
b2b0fa9a79049e6f5621e837ed4836919c6cf82dece4f60c93a30b12a3dbd400
5f0d826ff827e7d94d07bc9ee74d0a88c79bcf75bb024f05043486e1cbe294bd
O=S(=O)(c1ccccc1)n1ccc2cc(-c3ccccc3)ccc21
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[c:7]:[c:8]1:[c:9]:[c:10]:[c:11]:[nH;D2;+0:12]:1>>[O;D1;H0:2]=[S;H0;D4;+0:1](=[O;D1;H0:3])(-[c:4](:[c:5]):[c:6])-[n;H0;D3;+0:12]1:[c:11]:[c:10]:[c:9]:[c:8]:1:[c:7]
42.2
[{"value": 42.2, "product": "C1(=CC=CC=C1)S(=O)(=O)N1C=CC2=CC(=CC=C12)C1=CC(=CC=C1)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To a stirred slurry of 0.61 g (12.7 mmol), 50% dispersion of NaH in mineral oil, in 36 mL anhydrous THF was added 2.15 g crude 5-(3-chlorophenyl)indole (Step 1 of Example 45). The solution was allowed to stir at room temperature 15 min upon which time 1.2 mL (9.4 mmol) phenylsulfonyl chloride was added dropwise. The so...
10.6084/m9.figshare.5104873.v1
null
Sulfonyl halide
null
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
c1ccccc1.c1ccc2[nH]ccc2c1.c1ccccc1
HCl
C1CCOC1
null
8
Clc1cccc(-c2ccc3[nH]ccc3c2)c1.O=S(=O)(Cl)c1ccccc1>C1CCOC1>O=S(=O)(c1ccccc1)n1ccc2cc(-c3cccc(Cl)c3)ccc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-fea3f796f3cd4a8cb293301673c4d261
O=S(=O)(c1ccccc1)n1ccc2cc(-c3cccc(Cl)c3)ccc21.OC1CCCC1>>Clc1cccc(-c2ccc3c(ccn3C3CCCC3)c2)c1
CC(C)(C)[O-].[K+].C1(CCCC1)O.C1(=CC=CC=C1)S(=O)(=O)N1C=CC2=CC(=CC=C12)C1=CC(=CC=C1)Cl>>ClC=1C=C(C=CC1)C=1C=C2C=CN(C2=CC1)C1CCCC1
O=S(=O)(c1ccccc1)[n:14]1[c:10]2[cH:9][cH:8][c:7](-[c:6]3[cH:5][cH:4][cH:3][c:2]([Cl:1])[cH:21]3)[cH:20][c:11]2[cH:12][cH:13]1.O[CH:15]1[CH2:16][CH2:17][CH2:18][CH2:19]1>>[Cl:1][c:2]1[cH:3][cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]3[c:11]([cH:12][cH:13][n:14]3[CH:15]3[CH2:16][CH2:17][CH2:18][CH2:19]3)[cH:20]2)[cH:21]1
O=S(=O)(c1ccccc1)n1ccc2cc(-c3cccc(Cl)c3)ccc21.OC1CCCC1
Clc1cccc(-c2ccc3c(ccn3C3CCCC3)c2)c1
null
null
[Cl-].[Na+].O.C1(=CC=CC=C1)C.C1CCOC1
Heteroatom Alkylation and Arylation
OtherReaction
6c63ad0e43571b718b9bb9b22f2e8ed127a9af6ff3894c292116211cd0b45762
7e4920259a1416b2ad82882dcdd5ff78bfba80ea8d17566c27d0d8f23a71cd94
c1ccc(-c2ccc3c(ccn3C3CCCC3)c2)cc1
O-[CH;D3;+0:1]1-[C:2]-[C:3]-[C:4]-[C:5]-1.O=S(=O)(-[n;H0;D3;+0:6]1:[c:7]:[c:8]:[c:9]:[c:10]:1:[c:11])-c1:c:c:c:c:c:1>>[c:11]:[c:10]1:[c:9]:[c:8]:[c:7]:[n;H0;D3;+0:6]:1-[CH;D3;+0:1]1-[C:2]-[C:3]-[C:4]-[C:5]-1
null
[]
150
CELSIUS
null
null
A 5 mL conical glass microwave reaction vessel with stir bar, sealed with a septum and swept with nitrogen, was charged with a solution of 0.08 g (0.22 mmol) 1-(benzenesulfonyl-5-(3-chlorophenyl)-1H-indole in 1.2 mL anhydrous toluene. 32 μL (0.33 mmol) cyclopentanol was added with stirring, followed by 0.3 mL 1.0 M sol...
10.6084/m9.figshare.5104873.v1
null
Secondary alcohol
null
c1ccccc1.c1ccc2[nH]ccc2c1.C1CCCC1
c1ccc2[nH]ccc2c1.C1CCCC1
c1ccccc1.c1ccc2[nH]ccc2c1.C1CCCC1
HO-
[Cl-].[Na+].O.C1(=CC=CC=C1)C.C1CCOC1
150
null
O=S(=O)(c1ccccc1)n1ccc2cc(-c3cccc(Cl)c3)ccc21.OC1CCCC1>[Cl-].[Na+].O.C1(=CC=CC=C1)C.C1CCOC1>Clc1cccc(-c2ccc3c(ccn3C3CCCC3)c2)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-611af92e7dae4267bc90a76f838d59bc
Clc1cccc(-c2ccc3c(ccn3C3CCCC3)c2)c1.O=C(Cl)C(=O)Cl>>O=C(O)C(=O)c1cn(C2CCCC2)c2ccc(-c3cccc(Cl)c3)cc12
ClC=1C=C(C=CC1)C=1C=C2C=CN(C2=CC1)C1CCCC1.C1CCOC1.C(=O)(C(=O)Cl)Cl>>ClC=1C=C(C=CC1)C=1C=C2C(=CN(C2=CC1)C1CCCC1)C(C(=O)O)=O
[cH:6]1[cH:7][n:8]([CH:9]2[CH2:10][CH2:11][CH2:12][CH2:13]2)[c:14]2[cH:15][cH:16][c:17](-[c:18]3[cH:19][cH:20][cH:21][c:22]([Cl:23])[cH:24]3)[cH:25][c:26]12.Cl[C:2](=[O:1])[C:4](Cl)=[O:5]>>[O:1]=[C:2]([OH:3])[C:4](=[O:5])[c:6]1[cH:7][n:8]([CH:9]2[CH2:10][CH2:11][CH2:12][CH2:13]2)[c:14]2[cH:15][cH:16][c:17](-[c:18]3[cH:...
Clc1cccc(-c2ccc3c(ccn3C3CCCC3)c2)c1.O=C(Cl)C(=O)Cl
O=C(O)C(=O)c1cn(C2CCCC2)c2ccc(-c3cccc(Cl)c3)cc12
null
null
null
Acylation
OtherReaction
9d127b05b36fe9fe6fc80547d3614a823e90d1399390b2ba6617beb8202d8432
6b048b617f07704989b0d7eff26dc61c44694ea4e42b339d6d7680e8458e5255
c1ccc(-c2ccc3c(ccn3C3CCCC3)c2)cc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C;H0;D3;+0:3](-Cl)=[O;D1;H0:4].[C:5]-[#7;a:6]1:[c:7]:[cH;D2;+0:8]:[c:9](:[c:10]):[c:11]:1:[c:12]>>[C:5]-[#7;a:6]1:[c:7]:[c;H0;D3;+0:8](-[C;H0;D3;+0:3](=[O;D1;H0:4])-[C;H0;D3;+0:1](=[O;D1;H0:2])-[O;D1;H1:13]):[c:9](:[c:10]):[c:11]:1:[c:12]
null
[]
null
null
null
null
The product from Step 3 of Example 45 was dissolved in 0.5 ml anhydrous THF and 50 μL (COCl)2 was added. The solution was mixed at room temperature overnight with orbital shaking. An aliquot removed for LC analysis indicated that the reaction was complete. The solution was added to 1 mL aqueous NaHCO3 and the vial was ...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Acyl halide
Carboxylic acid.Ketone
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
C1CCCC1.c1ccc2[nH]ccc2c1.c1ccccc1
Other
null
null
null
Clc1cccc(-c2ccc3c(ccn3C3CCCC3)c2)c1.O=C(Cl)C(=O)Cl>>O=C(O)C(=O)c1cn(C2CCCC2)c2ccc(-c3cccc(Cl)c3)cc12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-93b4e1e9211d4d059eda2a8ed161a707
Cn1ccc2ccc(-c3ccc(C(F)(F)F)cc3)cc21.O=C=O>>Cn1cc(C(=O)O)c2ccc(-c3ccc(C(F)(F)F)cc3)cc21
C(=O)=O.CN1C=CC2=CC=C(C=C12)C1=CC=C(C=C1)C(F)(F)F.C(CCC)[Li]>>CN1C=C(C2=CC=C(C=C12)C1=CC=C(C=C1)C(F)(F)F)C(=O)O
[CH3:1][n:2]1[cH:3][cH:4][c:8]2[cH:9][cH:10][c:11](-[c:12]3[cH:13][cH:14][c:15]([C:16]([F:17])([F:18])[F:19])[cH:20][cH:21]3)[cH:22][c:23]12.[C:5](=[O:6])=[O:7]>>[CH3:1][n:2]1[cH:3][c:4]([C:5](=[O:6])[OH:7])[c:8]2[cH:9][cH:10][c:11](-[c:12]3[cH:13][cH:14][c:15]([C:16]([F:17])([F:18])[F:19])[cH:20][cH:21]3)[cH:22][c:23]...
Cn1ccc2ccc(-c3ccc(C(F)(F)F)cc3)cc21.O=C=O
Cn1cc(C(=O)O)c2ccc(-c3ccc(C(F)(F)F)cc3)cc21
null
null
C1CCOC1
Acylation
OtherReaction
df7c74f2ca61ca5e8f920d60e8c90613bc2bb44892a91d0192b927d32b27b4ca
f2fa2063dd26da08ea200eb6cbb3037b91013a82352a2b60120e98f9e54cbd88
c1ccc(-c2ccc3cc[nH]c3c2)cc1
[C;D1;H3:1]-[#7;a:2]1:[c:3]:[cH;D2;+0:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[O;D1;H0:9]=[C;H0;D2;+0:10]=[O;H0;D1;+0:11]>>[C;D1;H3:1]-[#7;a:2]1:[c:3]:[c;H0;D3;+0:4](-[C;H0;D3;+0:10](=[O;D1;H0:9])-[OH;D1;+0:11]):[c:5](:[c:6]):[c:7]:1:[c:8]
19
[{"value": 19.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
-78
CELSIUS
30
MINUTE
To a solution of 1-methyl-6-(4-trifluoromethyl-phenyl)-1H-indole (0.483 g, 1.75 mmol) in dry THF (10 mL) at −78° C. was added n-butyllithium (0.84 mL, 2.1 mmol). The reaction mixture was stirred under nitrogen at −78° C. for 30 minutes then at −50 to −40° C. for 30 minutes. It reaction temperature was cooled to −78° C....
10.6084/m9.figshare.5104873.v1
null
Carbon dioxide
Carboxylic acid
c1ccc2cc[nH]c2c1
c1ccc2cc[nH]c2c1
c1ccc2cc[nH]c2c1.c1ccccc1
null
C1CCOC1
-78
0.5
Cn1ccc2ccc(-c3ccc(C(F)(F)F)cc3)cc21.O=C=O>C1CCOC1>Cn1cc(C(=O)O)c2ccc(-c3ccc(C(F)(F)F)cc3)cc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5ec2f35bd10448598046f7b4147eeb64
Cn1ccc2ccc(-c3ccc(C(C)(C)C)cc3)cc21.O=C=O>>Cn1cc(C(=O)O)c2ccc(-c3ccc(C(C)(C)C)cc3)cc21
C(C)(C)(C)C1=CC=C(C=C1)C1=CC=C2C=CN(C2=C1)C.C(CCC)[Li].C(=O)=O>>C(C)(C)(C)C1=CC=C(C=C1)C1=CC=C2C(=CN(C2=C1)C)C(=O)O
[CH3:1][n:2]1[cH:3][cH:4][c:8]2[cH:9][cH:10][c:11](-[c:12]3[cH:13][cH:14][c:15]([C:16]([CH3:17])([CH3:18])[CH3:19])[cH:20][cH:21]3)[cH:22][c:23]12.[C:5](=[O:6])=[O:7]>>[CH3:1][n:2]1[cH:3][c:4]([C:5](=[O:6])[OH:7])[c:8]2[cH:9][cH:10][c:11](-[c:12]3[cH:13][cH:14][c:15]([C:16]([CH3:17])([CH3:18])[CH3:19])[cH:20][cH:21]3)[...
Cn1ccc2ccc(-c3ccc(C(C)(C)C)cc3)cc21.O=C=O
Cn1cc(C(=O)O)c2ccc(-c3ccc(C(C)(C)C)cc3)cc21
null
null
C1CCOC1
Acylation
OtherReaction
df7c74f2ca61ca5e8f920d60e8c90613bc2bb44892a91d0192b927d32b27b4ca
f2fa2063dd26da08ea200eb6cbb3037b91013a82352a2b60120e98f9e54cbd88
c1ccc(-c2ccc3cc[nH]c3c2)cc1
[C;D1;H3:1]-[#7;a:2]1:[c:3]:[cH;D2;+0:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[O;D1;H0:9]=[C;H0;D2;+0:10]=[O;H0;D1;+0:11]>>[C;D1;H3:1]-[#7;a:2]1:[c:3]:[c;H0;D3;+0:4](-[C;H0;D3;+0:10](=[O;D1;H0:9])-[OH;D1;+0:11]):[c:5](:[c:6]):[c:7]:1:[c:8]
10.7
[{"value": 10.7, "product": "C(C)(C)(C)C1=CC=C(C=C1)C1=CC=C2C(=CN(C2=C1)C)C(=O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 10.7, "product": "C(C)(C)(C)C1=CC=C(C=C1)C1=CC=C2C(=CN(C2=C1)C)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
6-(4-tert-Butyl-phenyl)-1-methyl-1H-indole-3-carboxylic acid was prepared from 6-(4-tert-butyl-phenyl)-1-methyl-1H-indole (0.541 g, 2.05 mmol), n-butyllithium (0.98 mL, 2.5 mmol), crushed dry ice (3 g, 70 mmol) in dry THF (10 mL) according to the procedure described in Example 60. Purification by flash chromatography u...
10.6084/m9.figshare.5104873.v1
null
Carbon dioxide
Carboxylic acid
c1ccc2cc[nH]c2c1
c1ccc2cc[nH]c2c1
c1ccc2cc[nH]c2c1.c1ccccc1
null
C1CCOC1
null
null
Cn1ccc2ccc(-c3ccc(C(C)(C)C)cc3)cc21.O=C=O>C1CCOC1>Cn1cc(C(=O)O)c2ccc(-c3ccc(C(C)(C)C)cc3)cc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f2c14f61129d4978b91d83e4b3022efc
Fc1ccc(-c2ccc3c(ccn3Cc3ccccc3)c2)cc1Cl.O=C=O>>O=C(O)c1cn(Cc2ccccc2)c2ccc(-c3ccc(F)c(Cl)c3)cc12
C(C1=CC=CC=C1)N1C=CC2=CC(=CC=C12)C1=CC(=C(C=C1)F)Cl.C(CCC)[Li].C(=O)=O>>C(C1=CC=CC=C1)N1C=C(C2=CC(=CC=C12)C1=CC(=C(C=C1)F)Cl)C(=O)O
[cH:4]1[cH:5][n:6]([CH2:7][c:8]2[cH:9][cH:10][cH:11][cH:12][cH:13]2)[c:14]2[cH:15][cH:16][c:17](-[c:18]3[cH:19][cH:20][c:21]([F:22])[c:23]([Cl:24])[cH:25]3)[cH:26][c:27]12.[O:1]=[C:2]=[O:3]>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][n:6]([CH2:7][c:8]2[cH:9][cH:10][cH:11][cH:12][cH:13]2)[c:14]2[cH:15][cH:16][c:17](-[c:18]3[cH:19]...
Fc1ccc(-c2ccc3c(ccn3Cc3ccccc3)c2)cc1Cl.O=C=O
O=C(O)c1cn(Cc2ccccc2)c2ccc(-c3ccc(F)c(Cl)c3)cc12
null
null
C1CCOC1
Acylation
OtherReaction
73b6b50aa9b03f0c498dcfa29ca94d47bf015c87854538026c3079cdf775e6ac
f2fa2063dd26da08ea200eb6cbb3037b91013a82352a2b60120e98f9e54cbd88
c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
[C:1]-[#7;a:2]1:[c:3]:[cH;D2;+0:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[O;D1;H0:9]=[C;H0;D2;+0:10]=[O;H0;D1;+0:11]>>[C:1]-[#7;a:2]1:[c:3]:[c;H0;D3;+0:4](-[C;H0;D3;+0:10](=[O;D1;H0:9])-[OH;D1;+0:11]):[c:5](:[c:6]):[c:7]:1:[c:8]
32
[{"value": 32.0, "product": "C(C1=CC=CC=C1)N1C=C(C2=CC(=CC=C12)C1=CC(=C(C=C1)F)Cl)C(=O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 32.0, "product": "C(C1=CC=CC=C1)N1C=C(C2=CC(=CC=C12)C1=CC(=C(C=C1)F)Cl)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
1-Benzyl-5-(3-chloro-4-fluoro-phenyl)-1H-indole-3-carboxylic acid was prepared from 1-benzyl-5-(3-chloro-4-fluorophenyl)-1H-indole (17.99 g, 53.6 mmol), n-butyllithium (26 mL, 65 mmol), crushed dry ice (20 g, 450 mmol) in dry THF (180 mL) according to the procedure described in Example 60. Purification by HPLC using 85...
10.6084/m9.figshare.5104873.v1
null
Carbon dioxide
Carboxylic acid
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
c1ccccc1.c1ccc2[nH]ccc2c1.c1ccccc1
null
C1CCOC1
null
null
Fc1ccc(-c2ccc3c(ccn3Cc3ccccc3)c2)cc1Cl.O=C=O>C1CCOC1>O=C(O)c1cn(Cc2ccccc2)c2ccc(-c3ccc(F)c(Cl)c3)cc12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-9299ce90a014458f90c0ed8e50ecd9e9
Brc1ccc2[nH]ccc2c1.C=O.CNC>>CN(C)Cc1c[nH]c2ccc(Br)cc12
CNC.C=O.BrC=1C=C2C=CNC2=CC1>>BrC=1C=C2C(=CNC2=CC1)CN(C)C
[cH:5]1[cH:6][nH:7][c:8]2[cH:9][cH:10][c:11]([Br:12])[cH:13][c:14]12.O=[CH2:4].[CH3:1][NH:2][CH3:3]>>[CH3:1][N:2]([CH3:3])[CH2:4][c:5]1[cH:6][nH:7][c:8]2[cH:9][cH:10][c:11]([Br:12])[cH:13][c:14]12
Brc1ccc2[nH]ccc2c1.C=O.CNC
CN(C)Cc1c[nH]c2ccc(Br)cc12
null
null
C(C)(=O)O
Heteroatom Alkylation and Arylation
OtherReaction
14f2bfa3d907d463fab4dfc74293051dd668edd77fb6e0a45ccb47b35b91e990
e1fdef8fde1c506d7c9deb8fd5e6f322eceea2abce3167abcf412a1fa4fd5443
c1ccc2[nH]ccc2c1
O=[CH2;D1;+0:1].[C;D1;H3:2]-[NH;D2;+0:3]-[C;D1;H3:4].[c:5]:[c:6]1:[cH;D2;+0:7]:[c:8]:[#7;a:9]:[c:10]:1:[c:11]>>[C;D1;H3:2]-[N;H0;D3;+0:3](-[C;D1;H3:4])-[CH2;D2;+0:1]-[c;H0;D3;+0:7]1:[c:8]:[#7;a:9]:[c:10](:[c:11]):[c:6]:1:[c:5]
88.7
[{"value": 88.7, "product": "BrC=1C=C2C(=CNC2=CC1)CN(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
21
HOUR
To a mixture of 40% aqueous dimethylamine (5.95 g, 52.8 mmol), 37% aqueous formaldehyde (4.21 g, 51.9 mmol) and acetic acid (7 mL) was added 5-bromo-1H-indole (9.79 g, 49.9 mmol). The reaction mixture was stirred for 21 hours at room temperature and poured into a 2.5 N sodium hydroxide/ice mixture (200 mL). This was ex...
10.6084/m9.figshare.5104873.v1
null
Formaldehyde.Secondary amine
Tertiary amine
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
HO-
C(C)(=O)O
null
21
Brc1ccc2[nH]ccc2c1.C=O.CNC>C(C)(=O)O>CN(C)Cc1c[nH]c2ccc(Br)cc12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-76d2e0726b0d492a92d963f3bba1cef9
CN(C)Cc1c[nH]c2ccc(Br)cc12>>N#CCc1c[nH]c2ccc(Br)cc12
BrC=1C=C2C(=CNC2=CC1)CN(C)C.C[Si](C)(C)C#N.[F-].C(CCC)[N+](CCCC)(CCCC)CCCC.IC>>BrC=1C=C2C(=CNC2=CC1)CC#N
CN(C)[CH2:3][c:4]1[cH:5][nH:6][c:7]2[cH:8][cH:9][c:10]([Br:11])[cH:12][c:13]12>>[N:1]#[C:2][CH2:3][c:4]1[cH:5][nH:6][c:7]2[cH:8][cH:9][c:10]([Br:11])[cH:12][c:13]12
CN(C)Cc1c[nH]c2ccc(Br)cc12
N#CCc1c[nH]c2ccc(Br)cc12
null
null
C1=CC=CC=C1.O.C1CCOC1
Miscellaneous
OtherReaction
eeb390a765a14be516804ac95cf046d9e14d2a33610d749ac9b0df57ebee4fc2
dbf463487c354e590d1a121365b90aebc9d0a0d1f40f1a429596c4c6b1e08f52
c1ccc2[nH]ccc2c1
C-N(-C)-[CH2;D2;+0:1]-[c:2]1:[c:3]:[c:4]:[#7;a:5]:[c:6]:1>>[N;D1;H0:7]#[C:8]-[CH2;D2;+0:1]-[c:2]1:[c:3]:[c:4]:[#7;a:5]:[c:6]:1
51.1
[{"value": 51.0, "product": "BrC=1C=C2C(=CNC2=CC1)CC#N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 51.1, "product": "BrC=1C=C2C(=CNC2=CC1)CC#N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To an ice cooled suspension of (5-bromo-1H-indol-3-ylmethyl)-dimethyl-amine (11.2 g, 44.1 mmol) in benzene (145 mL) was added iodomethane (8.2 mL, 130 mmol). The reaction mixture was stirred overnight at room temperature and concentrated. The residue was dissolved in THF (210 mL). Trimethylsilyl cyanide (11.7 mL, 87.7 ...
10.6084/m9.figshare.5104873.v1
null
Tertiary amine
Nitrile
null
null
c1ccc2[nH]ccc2c1
Other
C1=CC=CC=C1.O.C1CCOC1
null
8
CN(C)Cc1c[nH]c2ccc(Br)cc12>C1=CC=CC=C1.O.C1CCOC1>N#CCc1c[nH]c2ccc(Br)cc12
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-072604a9467041429ec0d15ea0bffc5c
CI.N#CCc1c[nH]c2ccc(-c3ccc(C(F)(F)F)cc3)cc12>>Cn1cc(CC#N)c2cc(-c3ccc(C(F)(F)F)cc3)ccc21
FC(C1=CC=C(C=C1)C=1C=C2C(=CNC2=CC1)CC#N)(F)F.[H-].[Na+].IC>>CN1C=C(C2=CC(=CC=C12)C1=CC=C(C=C1)C(F)(F)F)CC#N
I[CH3:1].[nH:2]1[cH:3][c:4]([CH2:5][C:6]#[N:7])[c:8]2[cH:9][c:10](-[c:11]3[cH:12][cH:13][c:14]([C:15]([F:16])([F:17])[F:18])[cH:19][cH:20]3)[cH:21][cH:22][c:23]12>>[CH3:1][n:2]1[cH:3][c:4]([CH2:5][C:6]#[N:7])[c:8]2[cH:9][c:10](-[c:11]3[cH:12][cH:13][c:14]([C:15]([F:16])([F:17])[F:18])[cH:19][cH:20]3)[cH:21][cH:22][c:23...
CI.N#CCc1c[nH]c2ccc(-c3ccc(C(F)(F)F)cc3)cc12
Cn1cc(CC#N)c2cc(-c3ccc(C(F)(F)F)cc3)ccc21
null
null
C1CCOC1
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
5f4295751cbf2eac77c77b599ebb727e1800dd106de3a7476670f0ac76dbeba5
7a358c636daddc97c1fb4c29f378044d7eac3f01815d9966e599841f642d631a
c1ccc(-c2ccc3[nH]ccc3c2)cc1
I-[CH3;D1;+0:1].[c:2]:[c:3]1:[c:4]:[c:5]:[c:6]:[nH;D2;+0:7]:1>>[CH3;D1;+0:1]-[n;H0;D3;+0:7]1:[c:6]:[c:5]:[c:4]:[c:3]:1:[c:2]
60
[{"value": 60.0, "product": "CN1C=C(C2=CC(=CC=C12)C1=CC=C(C=C1)C(F)(F)F)CC#N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 59.8, "product": "CN1C=C(C2=CC(=CC=C12)C1=CC=C(C=C1)C(F)(F)F)CC#N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
[1-Methyl-5-(4-trifluoromethyl-phenyl)-1H-indol-3-yl]-acetonitrile was prepared from [5-(4-trifluoromethyl-phenyl)-1H-indol-3-yl]-acetonitrile (0.377 g, 1.26 mmol), sodium hydride (0.117 g, 2.93 mmol of a 60% dispersion on mineral oil), iodomethane ( 0.17 mL, 2.8 mmol) and THF (10 mL) according to the procedure describ...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.c1ccccc1
HI
C1CCOC1
null
null
CI.N#CCc1c[nH]c2ccc(-c3ccc(C(F)(F)F)cc3)cc12>C1CCOC1>Cn1cc(CC#N)c2cc(-c3ccc(C(F)(F)F)cc3)ccc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-3f3e8c19a7c34e0fbbd45aff63378f4c
Cc1cccc(-c2ccc3c(c2)c(C(=O)C(=O)O)cn3Cc2ccc(C(C)(C)C)cc2)c1>>Cc1cccc(-c2ccc3c(c2)c(CC(=O)O)cn3Cc2ccc(C(C)(C)C)cc2)c1
O.NN.C(C)(C)(C)C1=CC=C(CN2C=C(C3=CC(=CC=C23)C2=CC(=CC=C2)C)C(C(=O)O)=O)C=C1.C[O-].[Na+]>>C(C)(C)(C)C1=CC=C(CN2C=C(C3=CC(=CC=C23)C2=CC(=CC=C2)C)CC(=O)O)C=C1
O=[C:14]([c:13]1[c:11]2[c:10]([cH:9][cH:8][c:7](-[c:6]3[cH:5][cH:4][cH:3][c:2]([CH3:1])[cH:31]3)[cH:12]2)[n:19]([CH2:20][c:21]2[cH:22][cH:23][c:24]([C:25]([CH3:26])([CH3:27])[CH3:28])[cH:29][cH:30]2)[cH:18]1)[C:15](=[O:16])[OH:17]>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]3[c:11]([cH:12]2)[c:13]([C...
Cc1cccc(-c2ccc3c(c2)c(C(=O)C(=O)O)cn3Cc2ccc(C(C)(C)C)cc2)c1
Cc1cccc(-c2ccc3c(c2)c(CC(=O)O)cn3Cc2ccc(C(C)(C)C)cc2)c1
null
null
COCCO
Reduction
OtherReaction
bdac4f77103f4da1c5b42ea95e05b0b7b31176b78204db5f4144ffca7b3d54d5
f9ba67182f94acd5fbe41487f8f71e26bccf898b8fc8091ef46f4363de5628d4
c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
O=[C;H0;D3;+0:1](-[C:2](=[O;D1;H0:3])-[O;D1;H1:4])-[c:5]1:[c:6]:[c:7]:[#7;a:8](-[C:9]):[c:10]:1>>[C:9]-[#7;a:8]1:[c:7]:[c:6]:[c:5](-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[O;D1;H1:4]):[c:10]:1
46.7
[{"value": 46.7, "product": "C(C)(C)(C)C1=CC=C(CN2C=C(C3=CC(=CC=C23)C2=CC(=CC=C2)C)CC(=O)O)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
1
HOUR
Hydrazine monohydrate (0.56 mL, 11.75 mmol) was added to a stirring solution of 2-[1-[4-(tert-Butyl)benzyl]-5-(3-methylphenyl)-1H-indol-3-yl]-2-oxoacetic acid (WAY-201417, 1.0 g, 2.35 mmol) in 2-methoxyethanol (10 mL). After the mixture was heated to 60° C. Sodium methoxide (1.34 g, 23.5 mmol) was added portionwise to ...
10.6084/m9.figshare.5104873.v1
null
Ketone
null
null
null
c1ccccc1.c1ccc2[nH]ccc2c1.c1ccccc1
Other
COCCO
60
1
Cc1cccc(-c2ccc3c(c2)c(C(=O)C(=O)O)cn3Cc2ccc(C(C)(C)C)cc2)c1>COCCO>Cc1cccc(-c2ccc3c(c2)c(CC(=O)O)cn3Cc2ccc(C(C)(C)C)cc2)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d6a90b55366546e79a79da13a90f1eb1
Cc1ccc(Cn2cc(C(=O)C(=O)O)c3cc(-c4ccc(OC(F)(F)F)cc4)ccc32)cc1>>Cc1ccc(Cn2cc(CC(=O)O)c3cc(-c4ccc(OC(F)(F)F)cc4)ccc32)cc1
CC1=CC=C(CN2C=C(C3=CC(=CC=C23)C2=CC=C(C=C2)OC(F)(F)F)C(C(=O)O)=O)C=C1.O.NN.C[O-].[Na+]>>CC1=CC=C(CN2C=C(C3=CC(=CC=C23)C2=CC=C(C=C2)OC(F)(F)F)CC(=O)O)C=C1
O=[C:10]([c:9]1[cH:8][n:7]([CH2:6][c:5]2[cH:4][cH:3][c:2]([CH3:1])[cH:32][cH:31]2)[c:30]2[c:14]1[cH:15][c:16](-[c:17]1[cH:18][cH:19][c:20]([O:21][C:22]([F:23])([F:24])[F:25])[cH:26][cH:27]1)[cH:28][cH:29]2)[C:11](=[O:12])[OH:13]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([CH2:6][n:7]2[cH:8][c:9]([CH2:10][C:11](=[O:12])[OH:13])[c:...
Cc1ccc(Cn2cc(C(=O)C(=O)O)c3cc(-c4ccc(OC(F)(F)F)cc4)ccc32)cc1
Cc1ccc(Cn2cc(CC(=O)O)c3cc(-c4ccc(OC(F)(F)F)cc4)ccc32)cc1
null
null
null
Reduction
OtherReaction
bdac4f77103f4da1c5b42ea95e05b0b7b31176b78204db5f4144ffca7b3d54d5
f9ba67182f94acd5fbe41487f8f71e26bccf898b8fc8091ef46f4363de5628d4
c1ccc(Cn2ccc3cc(-c4ccccc4)ccc32)cc1
O=[C;H0;D3;+0:1](-[C:2](=[O;D1;H0:3])-[O;D1;H1:4])-[c:5]1:[c:6]:[c:7]:[#7;a:8](-[C:9]):[c:10]:1>>[C:9]-[#7;a:8]1:[c:7]:[c:6]:[c:5](-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[O;D1;H1:4]):[c:10]:1
null
[]
null
null
null
null
The title compound was prepared from {1-(4-methylbenzyl)-5-[4-(trifluoromethoxy)phenyl]-1H-indol-3-yl}(oxo)acetic acid, hydrazine monohydrate and sodium methoxide according to the procedure described in Example 64. The product was obtained as a brown solid, mp: 62-63° C. Mass spectrum (−ESI, [M−H]−) m/z 438. 1HNMR (400...
10.6084/m9.figshare.5104873.v1
null
Ketone
null
null
null
c1ccccc1.c1ccc2[nH]ccc2c1.c1ccccc1
Other
null
null
null
Cc1ccc(Cn2cc(C(=O)C(=O)O)c3cc(-c4ccc(OC(F)(F)F)cc4)ccc32)cc1>>Cc1ccc(Cn2cc(CC(=O)O)c3cc(-c4ccc(OC(F)(F)F)cc4)ccc32)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0005d89300f14179ba31eec63084a118
COc1cc2c(Cl)ncnc2cc1OCCCN1CCOCC1.Oc1ccc2ncccc2c1>>COc1cc2c(Oc3ccc4ncccc4c3)ncnc2cc1OCCCN1CCOCC1
[OH-].[Na+].ClC1=NC=NC2=CC(=C(C=C12)OC)OCCCN1CCOCC1.C([O-])([O-])=O.[K+].[K+].OC=1C=C2C=CC=NC2=CC1>>COC=1C=C2C(=NC=NC2=CC1OCCCN1CCOCC1)OC=1C=C2C=CC=NC2=CC1
Cl[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:23]([O:24][CH2:25][CH2:26][CH2:27][N:28]3[CH2:29][CH2:30][O:31][CH2:32][CH2:33]3)[cH:22][c:21]2[n:20][cH:19][n:18]1.[OH:7][c:8]1[cH:9][cH:10][c:11]2[n:12][cH:13][cH:14][cH:15][c:16]2[cH:17]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([O:7][c:8]3[cH:9][cH:10][c:11]4[n:12][cH:13][cH:14...
COc1cc2c(Cl)ncnc2cc1OCCCN1CCOCC1.Oc1ccc2ncccc2c1
COc1cc2c(Oc3ccc4ncccc4c3)ncnc2cc1OCCCN1CCOCC1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
2d25b59c80a437134e7830160726da4e12ee4089c37759035843c1cccd8cd262
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1cnc2ccc(Oc3ncnc4cc(OCCCN5CCOCC5)ccc34)cc2c1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[OH;D1;+0:9]-[c:10](:[c:11]):[c:12]>>[c:11]:[c:10](-[O;H0;D2;+0:9]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8]):[c:12]
55
[{"value": 55.0, "product": "COC=1C=C2C(=NC=NC2=CC1OCCCN1CCOCC1)OC=1C=C2C=CC=NC2=CC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 54.5, "product": "COC=1C=C2C(=NC=NC2=CC1OCCCN1CCOCC1)OC=1C=C2C=CC=NC2=CC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
5
HOUR
A mixture of 4-chloro-6-methoxy-7-(3-morpholinopropoxy)quinazoline (225 mg, 0.67 mmol), potassium carbonate (106 mg, 0.77 mmol) and 6-hydroxyquinoline (112 mg, 0.77 mmol) in DMF (7.5 ml) was stirred at 100° C. for 5 hours and allowed to cool to ambient temperature. The reaction mixture was treated with 1M aqueous sodiu...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2ncccc2c1.c1ccc2ncncc2c1.C1COCC[NH]1
HCl
CN(C)C=O
100
5
COc1cc2c(Cl)ncnc2cc1OCCCN1CCOCC1.Oc1ccc2ncccc2c1>CN(C)C=O>COc1cc2c(Oc3ccc4ncccc4c3)ncnc2cc1OCCCN1CCOCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b4837dce22a34cdc876d8215b2e10c85
COc1cc(C(N)=O)c(N)cc1OCc1ccccc1>>COc1cc2c(=O)[nH]cnc2cc1OCc1ccccc1
NC1=C(C(=O)N)C=C(C(=C1)OCC1=CC=CC=C1)OC.CN(C)C=NC=[N+](C)C.[Cl-].C(C)(=O)[O-].[Na+].C(C)(=O)O>>C(C1=CC=CC=C1)OC1=C(C=C2C(NC=NC2=C1)=O)OC
[CH3:1][O:2][c:3]1[cH:4][c:5]([C:6](=[O:7])[NH2:8])[c:11]([NH2:10])[cH:12][c:13]1[O:14][CH2:15][c:16]1[cH:17][cH:18][cH:19][cH:20][cH:21]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6](=[O:7])[nH:8][cH:9][n:10][c:11]2[cH:12][c:13]1[O:14][CH2:15][c:16]1[cH:17][cH:18][cH:19][cH:20][cH:21]1
COc1cc(C(N)=O)c(N)cc1OCc1ccccc1
COc1cc2c(=O)[nH]cnc2cc1OCc1ccccc1
null
null
O1CCOCC1
Aromatic Heterocycle Formation
OtherReaction
0798449d56bc7e7756a703d33bd60780d26c4986e39e1809e15228456c95135b
3074b6c74bc99545969aa05d42dae7b149d9d6bb1b36a52cec3a362e1e7f7ca0
O=c1[nH]cnc2cc(OCc3ccccc3)ccc12
[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4](-[C;H0;D3;+0:5](-[NH2;D1;+0:6])=[O;D1;H0:7]):[c:8]>>[O;D1;H0:7]=[c;H0;D3;+0:5]1:[nH;D2;+0:6]:[c:9]:[n;H0;D2;+0:1]:[c:2](:[c:3]):[c:4]:1:[c:8]
84
[{"value": 84.0, "product": "C(C1=CC=CC=C1)OC1=C(C=C2C(NC=NC2=C1)=O)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 77.0, "product": "C(C1=CC=CC=C1)OC1=C(C=C2C(NC=NC2=C1)=O)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 2-amino-4-benzyloxy-5-methoxybenzamide (10 g, 0.04 mol), (J. Med. Chem. 1977, vol 20, 146–149), and Gold's reagent (7.4 g, 0.05 mol) in dioxane (100ml) was stirred and heated at reflux for 24 hours. Sodium acetate (3.02 g, 0.037 mol) and acetic acid (1.65 ml, 0.029 mol) were added to the reaction mixture a...
10.6084/m9.figshare.5104873.v1
null
Primary amide.Primary amine
null
c1ccccc1
c1ccc2ncncc2c1
c1ccc2ncncc2c1.c1ccccc1
Other
O1CCOCC1
null
null
COc1cc(C(N)=O)c(N)cc1OCc1ccccc1>O1CCOCC1>COc1cc2c(=O)[nH]cnc2cc1OCc1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f526d9d4190842b6bad655cc059ecc6a
COc1cc2c(=O)[nH]cnc2cc1OCc1ccccc1.O=S(Cl)Cl>>COc1cc2c(Cl)ncnc2cc1OCc1ccccc1
C(C1=CC=CC=C1)OC1=C(C=C2C(NC=NC2=C1)=O)OC.CN(C)C=O.S(=O)(Cl)Cl>>C(C1=CC=CC=C1)OC1=C(C=C2C(=NC=NC2=C1)Cl)OC
O=[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:13]([O:14][CH2:15][c:16]3[cH:17][cH:18][cH:19][cH:20][cH:21]3)[cH:12][c:11]2[n:10][cH:9][nH:8]1.O=S(Cl)[Cl:7]>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([Cl:7])[n:8][cH:9][n:10][c:11]2[cH:12][c:13]1[O:14][CH2:15][c:16]1[cH:17][cH:18][cH:19][cH:20][cH:21]1
COc1cc2c(=O)[nH]cnc2cc1OCc1ccccc1.O=S(Cl)Cl
COc1cc2c(Cl)ncnc2cc1OCc1ccccc1
null
null
null
Functional Group Interconversion
OtherReaction
3788560e87eee8765e749543914a91a512631307b97fad163ebef894d2a0ea68
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1ccc(COc2ccc3cncnc3c2)cc1
Cl-S(=O)-[Cl;H0;D1;+0:1].O=[c;H0;D3;+0:2]1:[nH;D2;+0:3]:[c:4]:[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9]>>[Cl;H0;D1;+0:1]-[c;H0;D3;+0:2]1:[n;H0;D2;+0:3]:[c:4]:[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9]
null
[]
null
null
null
null
7-Benzyloxy-6-methoxy-3,4-dihydroquinazolin-4-one (35 g, 124 mmol) was suspended in thionyl chloride (440 ml) and DMF (1.75 ml) and heated at reflux for 4 hours. The thionyl chloride was evaporated under vacuum and the residue azeotroped with toluene three times. The residue was dissolved in NMP (250 ml) to give a solu...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2ncncc2c1.c1ccccc1
HCl
null
null
null
COc1cc2c(=O)[nH]cnc2cc1OCc1ccccc1.O=S(Cl)Cl>>COc1cc2c(Cl)ncnc2cc1OCc1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-672212fe43174053a6b602a2597f9975
COc1cc2c(Cl)ncnc2cc1OCc1ccccc1.Oc1ccccc1>>COc1cc2c(Oc3ccccc3)ncnc2cc1OCc1ccccc1
O.[H-].[Na+].C1(=CC=CC=C1)O.C(C1=CC=CC=C1)OC1=C(C=C2C(=NC=NC2=C1)Cl)OC>>C(C1=CC=CC=C1)OC1=C(C=C2C(=NC=NC2=C1)OC1=CC=CC=C1)OC
Cl[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:19]([O:20][CH2:21][c:22]3[cH:23][cH:24][cH:25][cH:26][cH:27]3)[cH:18][c:17]2[n:16][cH:15][n:14]1.[OH:7][c:8]1[cH:9][cH:10][cH:11][cH:12][cH:13]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([O:7][c:8]3[cH:9][cH:10][cH:11][cH:12][cH:13]3)[n:14][cH:15][n:16][c:17]2[cH:18][c:19]1[O:20][CH...
COc1cc2c(Cl)ncnc2cc1OCc1ccccc1.Oc1ccccc1
COc1cc2c(Oc3ccccc3)ncnc2cc1OCc1ccccc1
null
null
CN1CCCC1=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
2d25b59c80a437134e7830160726da4e12ee4089c37759035843c1cccd8cd262
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1ccc(COc2ccc3c(Oc4ccccc4)ncnc3c2)cc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[OH;D1;+0:9]-[c:10](:[c:11]):[c:12]>>[c:11]:[c:10](-[O;H0;D2;+0:9]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8]):[c:12]
83
[{"value": 83.0, "product": "C(C1=CC=CC=C1)OC1=C(C=C2C(=NC=NC2=C1)OC1=CC=CC=C1)OC", "details": "PERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
Phenol (29.05 g, 309 mmol) was dissolved in NMP (210 ml), sodium hydride (11.025 g, 60% dispersion in mineral oil) was added in portions with cooling and the mixture was stirred for 3 hours. The viscous suspension was diluted with NMP (180 ml) and stirred overnight. The solution of 7-benzyloxy-4-chloro-6-methoxyquinazo...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccccc1.c1ccc2ncncc2c1.c1ccccc1
HCl
CN1CCCC1=O
null
3
COc1cc2c(Cl)ncnc2cc1OCc1ccccc1.Oc1ccccc1>CN1CCCC1=O>COc1cc2c(Oc3ccccc3)ncnc2cc1OCc1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-36e35b2dcbe54393ad2cd3b23febd9d7
COc1cc2c(Oc3ccccc3)ncnc2cc1OCc1ccccc1>>COc1cc2c(Oc3ccccc3)ncnc2cc1O
C(C1=CC=CC=C1)OC1=C(C=C2C(=NC=NC2=C1)OC1=CC=CC=C1)OC>>OC1=C(C=C2C(=NC=NC2=C1)OC1=CC=CC=C1)OC
c1ccc(C[O:20][c:19]2[c:3]([O:2][CH3:1])[cH:4][c:5]3[c:6]([O:7][c:8]4[cH:9][cH:10][cH:11][cH:12][cH:13]4)[n:14][cH:15][n:16][c:17]3[cH:18]2)cc1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([O:7][c:8]3[cH:9][cH:10][cH:11][cH:12][cH:13]3)[n:14][cH:15][n:16][c:17]2[cH:18][c:19]1[OH:20]
COc1cc2c(Oc3ccccc3)ncnc2cc1OCc1ccccc1
COc1cc2c(Oc3ccccc3)ncnc2cc1O
null
null
C(=O)(C(F)(F)F)O
Deprotection
Hydroxyl benzyl deprotection
36869d1fe85185a14d9eb30bf05178c600a9b6eca277ffaf3803578c30e0bf5d
26a36596df80ec137b0e8087297418351c93c32819177f680675220622f215d4
c1ccc(Oc2ncnc3ccccc23)cc1
[#7;a:1]:[c:2]:[c:3]:[c:4](-[O;H0;D2;+0:5]-C-c1:c:c:c:c:c:1):[c:6]>>[#7;a:1]:[c:2]:[c:3]:[c:4](-[OH;D1;+0:5]):[c:6]
96
[{"value": 96.0, "product": "OC1=C(C=C2C(=NC=NC2=C1)OC1=CC=CC=C1)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 94.0, "product": "OC1=C(C=C2C(=NC=NC2=C1)OC1=CC=CC=C1)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
7-Benzyloxy-6-methoxy-4-phenoxyquinazoline (36.95 g, 105.5 mmol) was suspended in TFA (420 ml) and heated at reflux for 3 hours. The reaction mixture was allowed to cool and evaporated under vacuum. The residue was stirred mechanically in water then basified with saturated aqueous sodium hydrogen carbonate solution and...
10.6084/m9.figshare.5104873.v1
null
Ether
Aromatic alcohol
c1ccccc1
null
c1ccccc1.c1ccc2ncncc2c1
Other
C(=O)(C(F)(F)F)O
null
null
COc1cc2c(Oc3ccccc3)ncnc2cc1OCc1ccccc1>C(=O)(C(F)(F)F)O>COc1cc2c(Oc3ccccc3)ncnc2cc1O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-67df1fd40f8a49ee96ddc5e8b3355166
C1COCCN1.ClCCCBr>>ClCCCN1CCOCC1
N1CCOCC1.BrCCCCl>>ClCCCN1CCOCC1
[NH:5]1[CH2:6][CH2:7][O:8][CH2:9][CH2:10]1.Br[CH2:4][CH2:3][CH2:2][Cl:1]>>[Cl:1][CH2:2][CH2:3][CH2:4][N:5]1[CH2:6][CH2:7][O:8][CH2:9][CH2:10]1
C1COCCN1.ClCCCBr
ClCCCN1CCOCC1
null
null
C1(=CC=CC=C1)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
2bad30dcdb0a20edb8ce877f072b133eedfd870621da393ec393128bfee00977
523d37155b42c8dc851abeddadebb241cdd90bdf649ba750c35e13c8c752d7b0
C1COCCN1
Br-[CH2;D2;+0:1]-[C:2]-[C:3].[#8:4]1-[C:5]-[C:6]-[NH;D2;+0:7]-[C:8]-[C:9]-1>>[C:3]-[C:2]-[CH2;D2;+0:1]-[N;H0;D3;+0:7]1-[C:8]-[C:9]-[#8:4]-[C:5]-[C:6]-1
77.2
[{"value": 77.0, "product": "ClCCCN1CCOCC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 77.2, "product": "ClCCCN1CCOCC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
70
CELSIUS
null
null
Morpholine (52.2 ml, 600 mmol) and 1-bromo-3-chloropropane (30 ml, 300 mmol) were dissolved in dry toluene (180 ml) and heated to 70° C. for 3 hours. The solid was removed by filtration and the filtrate evaporated under vacuum. The resulting oil was decanted from the additional solid residue and the oil was vacuum dist...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amine
Tertiary amine
C1COCCN1
C1COCC[NH]1
C1COCC[NH]1
HBr
C1(=CC=CC=C1)C
70
null
C1COCCN1.ClCCCBr>C1(=CC=CC=C1)C>ClCCCN1CCOCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-abe597ff8efa41fdb57f768e0a03584f
COc1cc2c(Oc3ccccc3)ncnc2cc1OCCCN1CCOCC1>>COc1cc2c(=O)[nH]cnc2cc1OCCCN1CCOCC1
COC=1C=C2C(=NC=NC2=CC1OCCCN1CCOCC1)OC1=CC=CC=C1>>COC=1C=C2C(NC=NC2=CC1OCCCN1CCOCC1)=O
c1ccc([O:7][c:6]2[c:5]3[cH:4][c:3]([O:2][CH3:1])[c:13]([O:14][CH2:15][CH2:16][CH2:17][N:18]4[CH2:19][CH2:20][O:21][CH2:22][CH2:23]4)[cH:12][c:11]3[n:10][cH:9][n:8]2)cc1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6](=[O:7])[nH:8][cH:9][n:10][c:11]2[cH:12][c:13]1[O:14][CH2:15][CH2:16][CH2:17][N:18]1[CH2:19][CH2:20][O:21][CH2:22][...
COc1cc2c(Oc3ccccc3)ncnc2cc1OCCCN1CCOCC1
COc1cc2c(=O)[nH]cnc2cc1OCCCN1CCOCC1
null
null
Cl
Miscellaneous
OtherReaction
35688e011295b3fd61af43341ada8b6a68d47734fb10ccd0734838342d415c85
291cad8b6dfbbd2c823b5c9d45efc37a166dc3454a9f151ac48cb357f4bc155f
O=c1[nH]cnc2cc(OCCCN3CCOCC3)ccc12
[c:1]:[c:2]1:[#7;a:3]:[c:4]:[n;H0;D2;+0:5]:[c;H0;D3;+0:6](-[O;H0;D2;+0:7]-c2:c:c:c:c:c:2):[c:8]:1:[c:9]>>[O;H0;D1;+0:7]=[c;H0;D3;+0:6]1:[nH;D2;+0:5]:[c:4]:[#7;a:3]:[c:2](:[c:1]):[c:8]:1:[c:9]
89.1
[{"value": 89.0, "product": "COC=1C=C2C(NC=NC2=CC1OCCCN1CCOCC1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 89.1, "product": "COC=1C=C2C(NC=NC2=CC1OCCCN1CCOCC1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
6-Methoxy-7-(3-morpholinopropoxy)-4-phenoxyquinazoline (33.08 g, 84 mmol) was dissolved in 6M aqueous hydrochloric acid (800 ml) and heated at reflux for 1.5 hours. The reaction mixture was decanted and concentrated to 250 ml then basified (pH9) with saturated aqueous sodium hydrogen carbonate solution. The aqueous lay...
10.6084/m9.figshare.5104873.v1
null
Ether
null
c1ccccc1.c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2ncncc2c1.C1COCC[NH]1
Other
Cl
null
null
COc1cc2c(Oc3ccccc3)ncnc2cc1OCCCN1CCOCC1>Cl>COc1cc2c(=O)[nH]cnc2cc1OCCCN1CCOCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c5247d25e4c64561a536322973f5e5ef
COc1cc2c(=O)[nH]cnc2cc1OCCCN1CCOCC1.O=S(Cl)Cl>>COc1cc2c(Cl)ncnc2cc1OCCCN1CCOCC1
COC=1C=C2C(NC=NC2=CC1OCCCN1CCOCC1)=O.CN(C)C=O.S(=O)(Cl)Cl>>ClC1=NC=NC2=CC(=C(C=C12)OC)OCCCN1CCOCC1
O=[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:13]([O:14][CH2:15][CH2:16][CH2:17][N:18]3[CH2:19][CH2:20][O:21][CH2:22][CH2:23]3)[cH:12][c:11]2[n:10][cH:9][nH:8]1.O=S(Cl)[Cl:7]>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([Cl:7])[n:8][cH:9][n:10][c:11]2[cH:12][c:13]1[O:14][CH2:15][CH2:16][CH2:17][N:18]1[CH2:19][CH2:20][O:21][CH2:22]...
COc1cc2c(=O)[nH]cnc2cc1OCCCN1CCOCC1.O=S(Cl)Cl
COc1cc2c(Cl)ncnc2cc1OCCCN1CCOCC1
null
null
null
Functional Group Interconversion
OtherReaction
3788560e87eee8765e749543914a91a512631307b97fad163ebef894d2a0ea68
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1ncc2ccc(OCCCN3CCOCC3)cc2n1
Cl-S(=O)-[Cl;H0;D1;+0:1].O=[c;H0;D3;+0:2]1:[nH;D2;+0:3]:[c:4]:[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9]>>[Cl;H0;D1;+0:1]-[c;H0;D3;+0:2]1:[n;H0;D2;+0:3]:[c:4]:[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9]
52
[{"value": 52.0, "product": "ClC1=NC=NC2=CC(=C(C=C12)OC)OCCCN1CCOCC1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
6-Methoxy-7-(3-morpholinopropoxy)-3,4-dihydroquinazolin-4-one (23.9 g, 75 mmol) was suspended in thionyl chloride (210 ml) and DMF (1.8 ml) then heated at reflux for 1.5 hours. The thionyl chloride was removed by evaporation under vacuum and the residue azeotroped with toluene three times. The residue was taken up in w...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2ncncc2c1.C1COCC[NH]1
HCl
null
null
null
COc1cc2c(=O)[nH]cnc2cc1OCCCN1CCOCC1.O=S(Cl)Cl>>COc1cc2c(Cl)ncnc2cc1OCCCN1CCOCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-3b09a4491fb64908b3138363b9488451
COc1cc2c(Cl)ncnc2cc1OCCCN1CCOCC1.Oc1ccc2cccnc2c1>>COc1cc2c(Oc3ccc4cccnc4c3)ncnc2cc1OCCCN1CCOCC1
[OH-].[Na+].ClC1=NC=NC2=CC(=C(C=C12)OC)OCCCN1CCOCC1.C([O-])([O-])=O.[K+].[K+].OC1=CC=C2C=CC=NC2=C1>>COC=1C=C2C(=NC=NC2=CC1OCCCN1CCOCC1)OC1=CC=C2C=CC=NC2=C1
Cl[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:23]([O:24][CH2:25][CH2:26][CH2:27][N:28]3[CH2:29][CH2:30][O:31][CH2:32][CH2:33]3)[cH:22][c:21]2[n:20][cH:19][n:18]1.[OH:7][c:8]1[cH:9][cH:10][c:11]2[cH:12][cH:13][cH:14][n:15][c:16]2[cH:17]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([O:7][c:8]3[cH:9][cH:10][c:11]4[cH:12][cH:13][cH:1...
COc1cc2c(Cl)ncnc2cc1OCCCN1CCOCC1.Oc1ccc2cccnc2c1
COc1cc2c(Oc3ccc4cccnc4c3)ncnc2cc1OCCCN1CCOCC1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
2d25b59c80a437134e7830160726da4e12ee4089c37759035843c1cccd8cd262
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1cnc2cc(Oc3ncnc4cc(OCCCN5CCOCC5)ccc34)ccc2c1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[#7;a:9]:[c:10]:[c:11]:[c:12](-[OH;D1;+0:13]):[c:14]>>[#7;a:9]:[c:10]:[c:11]:[c:12](-[O;H0;D2;+0:13]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8]):[c:14]
39
[{"value": 39.0, "product": "COC=1C=C2C(=NC=NC2=CC1OCCCN1CCOCC1)OC1=CC=C2C=CC=NC2=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 38.8, "product": "COC=1C=C2C(=NC=NC2=CC1OCCCN1CCOCC1)OC1=CC=C2C=CC=NC2=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
5
HOUR
A mixture of 4-chloro-6-methoxy-7-(3-morpholinopropoxy)quinazoline (225 mg, 0.67 mmol), (prepared as described for the starting material in Example 1), potassium carbonate (106 g, 0.77 mmol) and 7-hydroxyquinoline (112 mg, 0.77 mmol) in DMF (7.5 ml) was stirred at 100° C. for 5 hours and allowed to cool to ambient temp...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2ncccc2c1.c1ccc2ncncc2c1.C1COCC[NH]1
HCl
CN(C)C=O
100
5
COc1cc2c(Cl)ncnc2cc1OCCCN1CCOCC1.Oc1ccc2cccnc2c1>CN(C)C=O>COc1cc2c(Oc3ccc4cccnc4c3)ncnc2cc1OCCCN1CCOCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-8f09a10886004035a4e54b16cdcc6b3a
COc1cc2c(Cl)ncnc2cc1OCCCN1CCOCC1.Oc1cccc2ccccc12>>COc1cc2c(Oc3cccc4ccccc34)ncnc2cc1OCCCN1CCOCC1
[OH-].[Na+].ClC1=NC=NC2=CC(=C(C=C12)OC)OCCCN1CCOCC1.C([O-])([O-])=O.[K+].[K+].C1(=CC=CC2=CC=CC=C12)O>>COC=1C=C2C(=NC=NC2=CC1OCCCN1CCOCC1)OC1=CC=CC2=CC=CC=C12
Cl[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:23]([O:24][CH2:25][CH2:26][CH2:27][N:28]3[CH2:29][CH2:30][O:31][CH2:32][CH2:33]3)[cH:22][c:21]2[n:20][cH:19][n:18]1.[OH:7][c:8]1[cH:9][cH:10][cH:11][c:12]2[cH:13][cH:14][cH:15][cH:16][c:17]12>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([O:7][c:8]3[cH:9][cH:10][cH:11][c:12]4[cH:13][cH:...
COc1cc2c(Cl)ncnc2cc1OCCCN1CCOCC1.Oc1cccc2ccccc12
COc1cc2c(Oc3cccc4ccccc34)ncnc2cc1OCCCN1CCOCC1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
2d25b59c80a437134e7830160726da4e12ee4089c37759035843c1cccd8cd262
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1ccc2c(Oc3ncnc4cc(OCCCN5CCOCC5)ccc34)cccc2c1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[OH;D1;+0:9]-[c:10](:[c:11]):[c:12]>>[c:11]:[c:10](-[O;H0;D2;+0:9]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8]):[c:12]
65
[{"value": 65.0, "product": "COC=1C=C2C(=NC=NC2=CC1OCCCN1CCOCC1)OC1=CC=CC2=CC=CC=C12", "details": "PERCENTYIELD", "is_desired": false}, {"value": 65.0, "product": "COC=1C=C2C(=NC=NC2=CC1OCCCN1CCOCC1)OC1=CC=CC2=CC=CC=C12", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
5
HOUR
A mixture of 4-chloro-6-methoxy-7-(3-morpholinopropoxy)quinazoline (225 mg, 0.67 mmol), (prepared as described for the starting material in Example 1), potassium carbonate (106 mg, 0.77 mmol) and 1-naphthol (111 mg, 0.77 mmol) in DMF (7.5 ml) was stirred at 100° C. for 5 hours then allowed to cool to ambient temperatur...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2ccccc2c1.c1ccc2ncncc2c1.C1COCC[NH]1
HCl
CN(C)C=O
100
5
COc1cc2c(Cl)ncnc2cc1OCCCN1CCOCC1.Oc1cccc2ccccc12>CN(C)C=O>COc1cc2c(Oc3cccc4ccccc34)ncnc2cc1OCCCN1CCOCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-19d86247b43c4c8da664f827b85e6008
COc1cc2c(Cl)ncnc2cc1OCCCN1CCOCC1.Cc1ccnc2cc(O)ccc12>>COc1cc2c(Oc3ccc4c(C)ccnc4c3)ncnc2cc1OCCCN1CCOCC1
[OH-].[Na+].ClC1=NC=NC2=CC(=C(C=C12)OC)OCCCN1CCOCC1.C([O-])([O-])=O.[K+].[K+].OC1=CC=C2C(=CC=NC2=C1)C>>COC=1C=C2C(=NC=NC2=CC1OCCCN1CCOCC1)OC1=CC=C2C(=CC=NC2=C1)C
Cl[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:24]([O:25][CH2:26][CH2:27][CH2:28][N:29]3[CH2:30][CH2:31][O:32][CH2:33][CH2:34]3)[cH:23][c:22]2[n:21][cH:20][n:19]1.[OH:7][c:8]1[cH:9][cH:10][c:11]2[c:12]([CH3:13])[cH:14][cH:15][n:16][c:17]2[cH:18]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([O:7][c:8]3[cH:9][cH:10][c:11]4[c:12]([CH...
COc1cc2c(Cl)ncnc2cc1OCCCN1CCOCC1.Cc1ccnc2cc(O)ccc12
COc1cc2c(Oc3ccc4c(C)ccnc4c3)ncnc2cc1OCCCN1CCOCC1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
2d25b59c80a437134e7830160726da4e12ee4089c37759035843c1cccd8cd262
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1cnc2cc(Oc3ncnc4cc(OCCCN5CCOCC5)ccc34)ccc2c1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[#7;a:9]:[c:10]:[c:11]:[c:12](-[OH;D1;+0:13]):[c:14]>>[#7;a:9]:[c:10]:[c:11]:[c:12](-[O;H0;D2;+0:13]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8]):[c:14]
57
[{"value": 57.0, "product": "COC=1C=C2C(=NC=NC2=CC1OCCCN1CCOCC1)OC1=CC=C2C(=CC=NC2=C1)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 56.7, "product": "COC=1C=C2C(=NC=NC2=CC1OCCCN1CCOCC1)OC1=CC=C2C(=CC=NC2=C1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
5
HOUR
A mixture of 4-chloro-6-methoxy-7-(3-morpholinopropoxy)quinazoline (225 mg, 0.67 mmol), (prepared as described for the starting material in Example 1), potassium carbonate (106 mg, 0.77 mmol) and 7-hydroxy-4-methylquinoline (122 mg, 0.77 mmol), (Chem. Berich. 1967, 100, 2077), in DMF (7.5 ml) was stirred at 100° C. for...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2ncccc2c1.c1ccc2ncncc2c1.C1COCC[NH]1
HCl
CN(C)C=O
100
5
COc1cc2c(Cl)ncnc2cc1OCCCN1CCOCC1.Cc1ccnc2cc(O)ccc12>CN(C)C=O>COc1cc2c(Oc3ccc4c(C)ccnc4c3)ncnc2cc1OCCCN1CCOCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b95c0f24fb5144c7b69042eedf25564a
COc1cc2c(Cl)ncnc2cc1OCCCN1CCS(=O)(=O)CC1.Oc1ccc2cccnc2c1>>COc1cc2c(Oc3ccc4cccnc4c3)ncnc2cc1OCCCN1CCS(=O)(=O)CC1
[OH-].[Na+].ClC1=NC=NC2=CC(=C(C=C12)OC)OCCCN1CCS(CC1)(=O)=O.C([O-])([O-])=O.[K+].[K+].OC1=CC=C2C=CC=NC2=C1>>O=S1(CCN(CC1)CCCOC1=C(C=C2C(=NC=NC2=C1)OC1=CC=C2C=CC=NC2=C1)OC)=O
Cl[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:23]([O:24][CH2:25][CH2:26][CH2:27][N:28]3[CH2:29][CH2:30][S:31](=[O:32])(=[O:33])[CH2:34][CH2:35]3)[cH:22][c:21]2[n:20][cH:19][n:18]1.[OH:7][c:8]1[cH:9][cH:10][c:11]2[cH:12][cH:13][cH:14][n:15][c:16]2[cH:17]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([O:7][c:8]3[cH:9][cH:10][c:11]4[...
COc1cc2c(Cl)ncnc2cc1OCCCN1CCS(=O)(=O)CC1.Oc1ccc2cccnc2c1
COc1cc2c(Oc3ccc4cccnc4c3)ncnc2cc1OCCCN1CCS(=O)(=O)CC1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
2d25b59c80a437134e7830160726da4e12ee4089c37759035843c1cccd8cd262
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
O=S1(=O)CCN(CCCOc2ccc3c(Oc4ccc5cccnc5c4)ncnc3c2)CC1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[#7;a:9]:[c:10]:[c:11]:[c:12](-[OH;D1;+0:13]):[c:14]>>[#7;a:9]:[c:10]:[c:11]:[c:12](-[O;H0;D2;+0:13]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8]):[c:14]
73
[{"value": 73.0, "product": "O=S1(CCN(CC1)CCCOC1=C(C=C2C(=NC=NC2=C1)OC1=CC=C2C=CC=NC2=C1)OC)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 72.7, "product": "O=S1(CCN(CC1)CCCOC1=C(C=C2C(=NC=NC2=C1)OC1=CC=C2C=CC=NC2=C1)OC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
5
HOUR
A mixture of 4-chloro-7-(3-(1,1-dioxothiomorpholino)propoxy)-6-methoxyquinazoline (220 mg, 0.57 mmol), potassium carbonate (106 mg, 0.77 mmol) and 7-hydroxyquinoline (111 mg, 0.76 mmol) in DMF (7.5 ml) was stirred at 100° C. for 5 hours then allowed to cool to ambient temperature. The reaction mixture was treated with ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2ncccc2c1.c1ccc2ncncc2c1.C1CSCC[NH]1
HCl
CN(C)C=O
100
5
COc1cc2c(Cl)ncnc2cc1OCCCN1CCS(=O)(=O)CC1.Oc1ccc2cccnc2c1>CN(C)C=O>COc1cc2c(Oc3ccc4cccnc4c3)ncnc2cc1OCCCN1CCS(=O)(=O)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-6e4a2e6d07af474dba1790077b8de6ed
COc1cc2c(=O)[nH]cnc2cc1OCc1ccccc1.O=S(Cl)Cl>>COc1cc2c(Cl)ncnc2cc1OCc1ccccc1
C(C1=CC=CC=C1)OC1=C(C=C2C(NC=NC2=C1)=O)OC.CN(C)C=O.S(=O)(Cl)Cl>>C(C1=CC=CC=C1)OC1=C(C=C2C(=NC=NC2=C1)Cl)OC
O=[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:13]([O:14][CH2:15][c:16]3[cH:17][cH:18][cH:19][cH:20][cH:21]3)[cH:12][c:11]2[n:10][cH:9][nH:8]1.O=S(Cl)[Cl:7]>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([Cl:7])[n:8][cH:9][n:10][c:11]2[cH:12][c:13]1[O:14][CH2:15][c:16]1[cH:17][cH:18][cH:19][cH:20][cH:21]1
COc1cc2c(=O)[nH]cnc2cc1OCc1ccccc1.O=S(Cl)Cl
COc1cc2c(Cl)ncnc2cc1OCc1ccccc1
null
null
null
Functional Group Interconversion
OtherReaction
3788560e87eee8765e749543914a91a512631307b97fad163ebef894d2a0ea68
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1ccc(COc2ccc3cncnc3c2)cc1
Cl-S(=O)-[Cl;H0;D1;+0:1].O=[c;H0;D3;+0:2]1:[nH;D2;+0:3]:[c:4]:[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9]>>[Cl;H0;D1;+0:1]-[c;H0;D3;+0:2]1:[n;H0;D2;+0:3]:[c:4]:[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9]
null
[]
null
null
null
null
7-Benzyloxy-6-methoxy-3,4-dihydroquinazolin-4-one (20.3 g, 124 mmol), (prepared as described for the starting material in Example 1), was taken up in thionyl chloride (440 ml) and DMF (1.75 ml) then heated at reflux for 4 hours. The thionyl chloride was evaporated under vacuum and the residue azeotroped with toluene th...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2ncncc2c1.c1ccccc1
HCl
null
null
null
COc1cc2c(=O)[nH]cnc2cc1OCc1ccccc1.O=S(Cl)Cl>>COc1cc2c(Cl)ncnc2cc1OCc1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c9a78dfb7663487fa2f53baeda49ab42
COc1cc2c(Cl)ncnc2cc1OCc1ccccc1.Oc1ccc(Cl)cc1F>>COc1cc2c(Oc3ccc(Cl)cc3F)ncnc2cc1OCc1ccccc1
O.C(C1=CC=CC=C1)OC1=C(C=C2C(=NC=NC2=C1)Cl)OC.C([O-])([O-])=O.[K+].[K+].ClC1=CC(=C(C=C1)O)F>>C(C1=CC=CC=C1)OC1=C(C=C2C(=NC=NC2=C1)OC1=C(C=C(C=C1)Cl)F)OC
Cl[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:21]([O:22][CH2:23][c:24]3[cH:25][cH:26][cH:27][cH:28][cH:29]3)[cH:20][c:19]2[n:18][cH:17][n:16]1.[OH:7][c:8]1[cH:9][cH:10][c:11]([Cl:12])[cH:13][c:14]1[F:15]>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([O:7][c:8]3[cH:9][cH:10][c:11]([Cl:12])[cH:13][c:14]3[F:15])[n:16][cH:17][n:18][c:1...
COc1cc2c(Cl)ncnc2cc1OCc1ccccc1.Oc1ccc(Cl)cc1F
COc1cc2c(Oc3ccc(Cl)cc3F)ncnc2cc1OCc1ccccc1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
2d25b59c80a437134e7830160726da4e12ee4089c37759035843c1cccd8cd262
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1ccc(COc2ccc3c(Oc4ccccc4)ncnc3c2)cc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[OH;D1;+0:9]-[c:10](:[c:11]):[c:12]>>[c:11]:[c:10](-[O;H0;D2;+0:9]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8]):[c:12]
76
[{"value": 76.0, "product": "C(C1=CC=CC=C1)OC1=C(C=C2C(=NC=NC2=C1)OC1=C(C=C(C=C1)Cl)F)OC", "details": "PERCENTYIELD", "is_desired": false}]
100
CELSIUS
5
HOUR
A mixture of the crude 7-benzyloxy-4-chloro-6-methoxyquinazoline, potassium carbonate (50 g, 362 mmol) and 4-chloro-2-fluorophenol (8.8 ml, 83 mmol) in DMF (500 ml) was stirred at 100° C. for 5 hours then allowed to cool to ambient temperature overnight. The reaction mixture was poured into water (21) and was stirred a...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccccc1.c1ccc2ncncc2c1.c1ccccc1
HCl
CN(C)C=O
100
5
COc1cc2c(Cl)ncnc2cc1OCc1ccccc1.Oc1ccc(Cl)cc1F>CN(C)C=O>COc1cc2c(Oc3ccc(Cl)cc3F)ncnc2cc1OCc1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ad22f7bf657a4e92a7fad388b17051f4
COc1cc2c(Oc3ccc(Cl)cc3F)ncnc2cc1OCc1ccccc1>>COc1cc2c(Oc3ccc(Cl)cc3F)ncnc2cc1O
C(C1=CC=CC=C1)OC1=C(C=C2C(=NC=NC2=C1)OC1=C(C=C(C=C1)Cl)F)OC.C1(=CC=CC=C1)C>>ClC1=CC(=C(OC2=NC=NC3=CC(=C(C=C23)OC)O)C=C1)F
c1ccc(C[O:22][c:21]2[c:3]([O:2][CH3:1])[cH:4][c:5]3[c:6]([O:7][c:8]4[cH:9][cH:10][c:11]([Cl:12])[cH:13][c:14]4[F:15])[n:16][cH:17][n:18][c:19]3[cH:20]2)cc1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([O:7][c:8]3[cH:9][cH:10][c:11]([Cl:12])[cH:13][c:14]3[F:15])[n:16][cH:17][n:18][c:19]2[cH:20][c:21]1[OH:22]
COc1cc2c(Oc3ccc(Cl)cc3F)ncnc2cc1OCc1ccccc1
COc1cc2c(Oc3ccc(Cl)cc3F)ncnc2cc1O
null
null
C(=O)(C(F)(F)F)O
Deprotection
Hydroxyl benzyl deprotection
36869d1fe85185a14d9eb30bf05178c600a9b6eca277ffaf3803578c30e0bf5d
26a36596df80ec137b0e8087297418351c93c32819177f680675220622f215d4
c1ccc(Oc2ncnc3ccccc23)cc1
[#7;a:1]:[c:2]:[c:3]:[c:4](-[O;H0;D2;+0:5]-C-c1:c:c:c:c:c:1):[c:6]>>[#7;a:1]:[c:2]:[c:3]:[c:4](-[OH;D1;+0:5]):[c:6]
1,999.3
[{"value": 1999.3, "product": "ClC1=CC(=C(OC2=NC=NC3=CC(=C(C=C23)OC)O)C=C1)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
7-Benzyloxy-4-(4-chloro-2-fluorophenoxy)-6-methoxyquinazoline (1.4 g, 3.4 mmol) was suspended in TFA (15 ml) and heated at reflux for 3 hours. The reaction mixture was allowed to cool, toluene was added and the volatiles were removed by evaporation under vacuum. The residue was triturated with ether and then acetone. T...
10.6084/m9.figshare.5104873.v1
null
Ether
Aromatic alcohol
c1ccccc1
null
c1ccccc1.c1ccc2ncncc2c1
Other
C(=O)(C(F)(F)F)O
null
null
COc1cc2c(Oc3ccc(Cl)cc3F)ncnc2cc1OCc1ccccc1>C(=O)(C(F)(F)F)O>COc1cc2c(Oc3ccc(Cl)cc3F)ncnc2cc1O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f34a995a35ed4900be5a3bf68a995419
C=CS(=O)(=O)C=C.NCCCO>>O=S1(=O)CCN(CCCO)CC1
NCCCO.C(=C)S(=O)(=O)C=C>>O=S1(CCN(CC1)CCCO)=O
[O:1]=[S:2](=[O:3])([CH:4]=[CH2:5])[CH:12]=[CH2:11].[NH2:6][CH2:7][CH2:8][CH2:9][OH:10]>>[O:1]=[S:2]1(=[O:3])[CH2:4][CH2:5][N:6]([CH2:7][CH2:8][CH2:9][OH:10])[CH2:11][CH2:12]1
C=CS(=O)(=O)C=C.NCCCO
O=S1(=O)CCN(CCCO)CC1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
97798d54365c4c593d15899edbd669dc532e6c6ab5378706898ea9faa974a532
cefc6df58e07d9b40193ef729e97b03e3cecc4f809d3df23d8c2c9918762ceb6
O=S1(=O)CCNCC1
[CH2;D1;+0:1]=[CH;D2;+0:2]-[#16:3](=[O;D1;H0:4])(=[O;D1;H0:5])-[CH;D2;+0:6]=[CH2;D1;+0:7].[C:8]-[C:9]-[NH2;D1;+0:10]>>[C:8]-[C:9]-[N;H0;D3;+0:10]1-[CH2;D2;+0:1]-[CH2;D2;+0:2]-[#16:3](=[O;D1;H0:4])(=[O;D1;H0:5])-[CH2;D2;+0:6]-[CH2;D2;+0:7]-1
90
[{"value": 90.0, "product": "O=S1(CCN(CC1)CCCO)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 49.3, "product": "O=S1(CCN(CC1)CCCO)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
110
CELSIUS
null
null
A mixture of 3-amino-1-propanol (650 μl, 8.4 mmol) and vinyl sulphone (1 g, 8.4 mmol) was heated at 110° C. for 45 minutes. The mixture was allowed to cool and was purified by column chromatography eluting with methylene chloride/methanol (95/5) to give 3-(1,1-dioxothiomorpholino)-1-propanol (800 mg, 90%). Conditions: ...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Vinyl.Vinyl
Tertiary amine
null
C1CSCC[NH]1
C1CSCC[NH]1
null
null
110
null
C=CS(=O)(=O)C=C.NCCCO>>O=S1(=O)CCN(CCCO)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d77ca0f9e0534ccab0157a4494ac4df6
COc1cc2c(Oc3ccc(Cl)cc3F)ncnc2cc1O.O=S1(=O)CCN(CCCO)CC1>>COc1cc2c(Oc3ccc(Cl)cc3F)ncnc2cc1OCCCN1CCS(=O)(=O)CC1
N(=NC(=O)N1CCCCC1)C(=O)N1CCCCC1.ClC1=CC(=C(OC2=NC=NC3=CC(=C(C=C23)OC)O)C=C1)F.C(CCC)P(CCCC)CCCC.O=S1(CCN(CC1)CCCO)=O>>ClC1=CC(=C(OC2=NC=NC3=CC(=C(C=C23)OC)OCCCN2CCS(CC2)(=O)=O)C=C1)F
[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([O:7][c:8]3[cH:9][cH:10][c:11]([Cl:12])[cH:13][c:14]3[F:15])[n:16][cH:17][n:18][c:19]2[cH:20][c:21]1[OH:22].O[CH2:23][CH2:24][CH2:25][N:26]1[CH2:27][CH2:28][S:29](=[O:30])(=[O:31])[CH2:32][CH2:33]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([O:7][c:8]3[cH:9][cH:10][c:11]([Cl:12])[cH:13][c:...
COc1cc2c(Oc3ccc(Cl)cc3F)ncnc2cc1O.O=S1(=O)CCN(CCCO)CC1
COc1cc2c(Oc3ccc(Cl)cc3F)ncnc2cc1OCCCN1CCS(=O)(=O)CC1
null
null
ClCCl.CCOCC
Heteroatom Alkylation and Arylation
Mitsunobu aryl ether
86bfb73617450d22f9456ed5ce4d96a73f1f8fc0c016bebae57fda68e2da86a2
2258bd14c3b5449b92dc09cf9fa522f88d5071b4af20f7e968b60aa1ae6db0cf
O=S1(=O)CCN(CCCOc2ccc3c(Oc4ccccc4)ncnc3c2)CC1
O-[CH2;D2;+0:1]-[C:2]-[C:3].[#7;a:4]:[c:5]:[c:6]:[c:7](-[OH;D1;+0:8]):[c:9]>>[#7;a:4]:[c:5]:[c:6]:[c:7](-[O;H0;D2;+0:8]-[CH2;D2;+0:1]-[C:2]-[C:3]):[c:9]
70
[{"value": 70.0, "product": "ClC1=CC(=C(OC2=NC=NC3=CC(=C(C=C23)OC)OCCCN2CCS(CC2)(=O)=O)C=C1)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 69.8, "product": "ClC1=CC(=C(OC2=NC=NC3=CC(=C(C=C23)OC)OCCCN2CCS(CC2)(=O)=O)C=C1)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
4-(4-Chloro-2-fluorophenoxy)-7-hydroxy-6-methoxyquinazoline (5.0 g, 15.6 mmol) was suspended in dichloromethane (150 ml) and tributylphosphine (11.1 ml, 44.6 mmol) was added followed by stirring at ambient temperature for 30 minutes. To this mixture was added 3-(1,1-dioxothiomorpholino)-1-propanol (4.2 g, 21.8 mmol) fo...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Aromatic alcohol
Ether
null
null
c1ccccc1.c1ccc2ncncc2c1.C1CSCC[NH]1
HO-
ClCCl.CCOCC
null
0.5
COc1cc2c(Oc3ccc(Cl)cc3F)ncnc2cc1O.O=S1(=O)CCN(CCCO)CC1>ClCCl.CCOCC>COc1cc2c(Oc3ccc(Cl)cc3F)ncnc2cc1OCCCN1CCS(=O)(=O)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c918506e6f194ea3828b100f13b83d54
COc1cc2c(Oc3ccc(Cl)cc3F)ncnc2cc1OCCCN1CCS(=O)(=O)CC1>>COc1cc2c(=O)[nH]cnc2cc1OCCCN1CCS(=O)(=O)CC1
ClC1=CC(=C(OC2=NC=NC3=CC(=C(C=C23)OC)OCCCN2CCS(CC2)(=O)=O)C=C1)F.C(O)([O-])=O.[Na+]>>O=S1(CCN(CC1)CCCOC1=C(C=C2C(NC=NC2=C1)=O)OC)=O
Fc1cc(Cl)ccc1[O:7][c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:13]([O:14][CH2:15][CH2:16][CH2:17][N:18]3[CH2:19][CH2:20][S:21](=[O:22])(=[O:23])[CH2:24][CH2:25]3)[cH:12][c:11]2[n:10][cH:9][n:8]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6](=[O:7])[nH:8][cH:9][n:10][c:11]2[cH:12][c:13]1[O:14][CH2:15][CH2:16][CH2:17][N:18]1[CH2:19][C...
COc1cc2c(Oc3ccc(Cl)cc3F)ncnc2cc1OCCCN1CCS(=O)(=O)CC1
COc1cc2c(=O)[nH]cnc2cc1OCCCN1CCS(=O)(=O)CC1
null
null
Cl.O
Functional Group Interconversion
OtherReaction
2e331e7f987e2f208a7bb6621e9b7dc6ca9e78c94b181dc5496a50196c7c48fe
a99fd2343850f6fbc4a4d7024846a70661aad8ef3f77938589a06d4940f99c06
O=c1[nH]cnc2cc(OCCCN3CCS(=O)(=O)CC3)ccc12
Cl-c1:c:c:c(-[O;H0;D2;+0:1]-[c;H0;D3;+0:2]2:[n;H0;D2;+0:3]:[c:4]:[#7;a:5]:[c:6](:[c:7]):[c:8]:2:[c:9]):c(-F):c:1>>[O;H0;D1;+0:1]=[c;H0;D3;+0:2]1:[nH;D2;+0:3]:[c:4]:[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9]
87.9
[{"value": 87.0, "product": "O=S1(CCN(CC1)CCCOC1=C(C=C2C(NC=NC2=C1)=O)OC)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 87.9, "product": "O=S1(CCN(CC1)CCCOC1=C(C=C2C(NC=NC2=C1)=O)OC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
95
CELSIUS
null
null
4-(4-Chloro-2-fluorophenoxy)-7-(3-(1,1-dioxothiomorpholino)propoxy)-6-methoxyquinazoline (3.5 g, 7 mmol) was dissolved in 2M aqueous hydrochloric acid (56 ml) and heated at 95° C. for 2 hours. The cooled reaction mixture was treated with solid sodium hydrogen carbonate solution to give a thick paste which was diluted w...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide.Ether
null
c1ccccc1.c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2ncncc2c1.C1CSCC[NH]1
HF
Cl.O
95
null
COc1cc2c(Oc3ccc(Cl)cc3F)ncnc2cc1OCCCN1CCS(=O)(=O)CC1>Cl.O>COc1cc2c(=O)[nH]cnc2cc1OCCCN1CCS(=O)(=O)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-2f235a95498b4d10814564c5c2d79684
COc1cc2c(=O)[nH]cnc2cc1OCCCN1CCS(=O)(=O)CC1.O=S(Cl)Cl>>COc1cc2c(Cl)ncnc2cc1OCCCN1CCS(=O)(=O)CC1
O=S1(CCN(CC1)CCCOC1=C(C=C2C(NC=NC2=C1)=O)OC)=O.CN(C)C=O.S(=O)(Cl)Cl>>ClC1=NC=NC2=CC(=C(C=C12)OC)OCCCN1CCS(CC1)(=O)=O
O=[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:13]([O:14][CH2:15][CH2:16][CH2:17][N:18]3[CH2:19][CH2:20][S:21](=[O:22])(=[O:23])[CH2:24][CH2:25]3)[cH:12][c:11]2[n:10][cH:9][nH:8]1.O=S(Cl)[Cl:7]>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([Cl:7])[n:8][cH:9][n:10][c:11]2[cH:12][c:13]1[O:14][CH2:15][CH2:16][CH2:17][N:18]1[CH2:19][CH2...
COc1cc2c(=O)[nH]cnc2cc1OCCCN1CCS(=O)(=O)CC1.O=S(Cl)Cl
COc1cc2c(Cl)ncnc2cc1OCCCN1CCS(=O)(=O)CC1
null
null
C1(=CC=CC=C1)C
Functional Group Interconversion
OtherReaction
3788560e87eee8765e749543914a91a512631307b97fad163ebef894d2a0ea68
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
O=S1(=O)CCN(CCCOc2ccc3cncnc3c2)CC1
Cl-S(=O)-[Cl;H0;D1;+0:1].O=[c;H0;D3;+0:2]1:[nH;D2;+0:3]:[c:4]:[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9]>>[Cl;H0;D1;+0:1]-[c;H0;D3;+0:2]1:[n;H0;D2;+0:3]:[c:4]:[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9]
52
[{"value": 52.0, "product": "ClC1=NC=NC2=CC(=C(C=C12)OC)OCCCN1CCS(CC1)(=O)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
7-(3-(1, 1-Dioxothiomorpholino)propoxy)-6-methoxy-3,4-dihydroquinazolin-4-one (4.2 g, 11.4 mmol) was suspended in thionyl chloride (45 ml) and DMF (0.1 ml) then heated at reflux for 2.5 hours. The residue was diluted with toluene, the thionyl chloride was evaporated under vacuum, the residue was then azeotroped with to...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2ncncc2c1.C1CSCC[NH]1
HCl
C1(=CC=CC=C1)C
null
null
COc1cc2c(=O)[nH]cnc2cc1OCCCN1CCS(=O)(=O)CC1.O=S(Cl)Cl>C1(=CC=CC=C1)C>COc1cc2c(Cl)ncnc2cc1OCCCN1CCS(=O)(=O)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0c43765f9a3f4cde8df5f300566eb048
COc1cc2nc[nH]c(=O)c2cc1OC.O=S(Cl)Cl>>COc1cc2ncnc(Cl)c2cc1OC
COC=1C=C2C(NC=NC2=CC1OC)=O.S(=O)(Cl)Cl>>ClC1=NC=NC2=CC(=C(C=C12)OC)OC
O=[c:9]1[nH:8][cH:7][n:6][c:5]2[cH:4][c:3]([O:2][CH3:1])[c:13]([O:14][CH3:15])[cH:12][c:11]21.O=S(Cl)[Cl:10]>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8][c:9]([Cl:10])[c:11]2[cH:12][c:13]1[O:14][CH3:15]
COc1cc2nc[nH]c(=O)c2cc1OC.O=S(Cl)Cl
COc1cc2ncnc(Cl)c2cc1OC
null
CN(C)C=O
null
Functional Group Interconversion
OtherReaction
3788560e87eee8765e749543914a91a512631307b97fad163ebef894d2a0ea68
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1ccc2ncncc2c1
Cl-S(=O)-[Cl;H0;D1;+0:1].O=[c;H0;D3;+0:2]1:[nH;D2;+0:3]:[c:4]:[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9]>>[Cl;H0;D1;+0:1]-[c;H0;D3;+0:2]1:[n;H0;D2;+0:3]:[c:4]:[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9]
null
[]
null
null
null
null
6,7-Dimethoxy-3,4-dihydroquinazolin-4-one (290 mg, 1.4 mmol) was suspended in thionyl chloride (5 ml) and DMF (2 drops) and heated at reflux for 2 hours. The thionyl chloride was evaporated under vacuum and the residue azeotroped with toluene three times to give 4-chloro-6,7-dimethoxyquinazoline. A mixture of the crude...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2ncncc2c1
HCl
CN(C)C=O
null
null
COc1cc2nc[nH]c(=O)c2cc1OC.O=S(Cl)Cl>CN(C)C=O>COc1cc2ncnc(Cl)c2cc1OC
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-37bbdc2f6f0a44189f2d09f7b653fc72
COc1cc2ncnc(Cl)c2cc1OC.Oc1ccc2cccnc2c1>>COc1cc2ncnc(Oc3ccc4cccnc4c3)c2cc1OC
[OH-].[Na+].ClC1=NC=NC2=CC(=C(C=C12)OC)OC.C([O-])([O-])=O.[K+].[K+].OC1=CC=C2C=CC=NC2=C1>>COC=1C=C2C(=NC=NC2=CC1OC)OC1=CC=C2C=CC=NC2=C1
Cl[c:9]1[n:8][cH:7][n:6][c:5]2[cH:4][c:3]([O:2][CH3:1])[c:23]([O:24][CH3:25])[cH:22][c:21]21.[OH:10][c:11]1[cH:12][cH:13][c:14]2[cH:15][cH:16][cH:17][n:18][c:19]2[cH:20]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][n:8][c:9]([O:10][c:11]3[cH:12][cH:13][c:14]4[cH:15][cH:16][cH:17][n:18][c:19]4[cH:20]3)[c:21]2[cH:22][c:23...
COc1cc2ncnc(Cl)c2cc1OC.Oc1ccc2cccnc2c1
COc1cc2ncnc(Oc3ccc4cccnc4c3)c2cc1OC
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
2d25b59c80a437134e7830160726da4e12ee4089c37759035843c1cccd8cd262
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1cnc2cc(Oc3ncnc4ccccc34)ccc2c1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[#7;a:9]:[c:10]:[c:11]:[c:12](-[OH;D1;+0:13]):[c:14]>>[#7;a:9]:[c:10]:[c:11]:[c:12](-[O;H0;D2;+0:13]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8]):[c:14]
24
[{"value": 24.0, "product": "COC=1C=C2C(=NC=NC2=CC1OC)OC1=CC=C2C=CC=NC2=C1", "details": "PERCENTYIELD", "is_desired": false}]
100
CELSIUS
5
HOUR
6,7-Dimethoxy-3,4-dihydroquinazolin-4-one (290 mg, 1.4 mmol) was suspended in thionyl chloride (5 ml) and DMF (2 drops) and heated at reflux for 2 hours. The thionyl chloride was evaporated under vacuum and the residue azeotroped with toluene three times to give 4-chloro-6,7-dimethoxyquinazoline. A mixture of the crude...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2ncncc2c1.c1ccc2ncccc2c1
HCl
CN(C)C=O
100
5
COc1cc2ncnc(Cl)c2cc1OC.Oc1ccc2cccnc2c1>CN(C)C=O>COc1cc2ncnc(Oc3ccc4cccnc4c3)c2cc1OC
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-6cd23c6db37a414ea12170b692f454ab
COc1cc(N)c(C(=O)O)cc1OC.NC=O>>COc1cc2nc[nH]c(=O)c2cc1OC
COC=1C=C(C(C(=O)O)=CC1OC)N.C(=O)N>>COC=1C=C2C(NC=NC2=CC1OC)=O
O[C:9](=[O:10])[c:11]1[c:5]([NH2:6])[cH:4][c:3]([O:2][CH3:1])[c:13]([O:14][CH3:15])[cH:12]1.O=[CH:7][NH2:8]>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[n:6][cH:7][nH:8][c:9](=[O:10])[c:11]2[cH:12][c:13]1[O:14][CH3:15]
COc1cc(N)c(C(=O)O)cc1OC.NC=O
COc1cc2nc[nH]c(=O)c2cc1OC
null
null
O
Aromatic Heterocycle Formation
OtherReaction
5215b2aebdf37498a4d4a87048f2b5a68a2aa2731f8695ccc5897fee02296c51
42d7d0d29a255bcbf4fdad9c0b39487d2cf609ac6796e99c9c033d59efbdbdc9
O=c1[nH]cnc2ccccc12
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[NH2;D1;+0:6]):[c:7].O=[CH;D2;+0:8]-[NH2;D1;+0:9]>>[O;D1;H0:2]=[c;H0;D3;+0:1]1:[nH;D2;+0:9]:[cH;D2;+0:8]:[n;H0;D2;+0:6]:[c:5](:[c:7]):[c:3]:1:[c:4]
null
[]
190
CELSIUS
3
HOUR
A mixture of 4,5-dimethoxyanthranilic acid (19.7 g) and formamide (10 ml) was stirred and heated at 190° C. for 5 hours. The mixture was allowed to cool to approximately 80° C. and water (50 ml) was added. The mixture was then allowed to stand at ambient temperature for 3 hours. The precipitate was collected by filtrat...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amide.Primary amine
null
c1ccccc1
c1ccc2ncncc2c1
c1ccc2ncncc2c1
HO-
O
190
3
COc1cc(N)c(C(=O)O)cc1OC.NC=O>O>COc1cc2nc[nH]c(=O)c2cc1OC
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a0c6379d14634e24819afeaf203f941c
CCOC(=O)[C@@H]1CCCNC1>>CCOC(=O)[C@@H]1CCCN(C)C1
[OH-].[Na+].C(=O)O.N1C[C@H](C(=O)OCC)CCC1.C(O)([O-])=O.[Na+]>>CN1C[C@@H](CCC1)C(=O)OCC
[CH3:1][CH2:2][O:3][C:4](=[O:5])[C@@H:6]1[CH2:7][CH2:8][CH2:9][NH:10][CH2:12]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[C@@H:6]1[CH2:7][CH2:8][CH2:9][N:10]([CH3:11])[CH2:12]1
CCOC(=O)[C@@H]1CCCNC1
CCOC(=O)[C@@H]1CCCN(C)C1
null
null
C=O
Miscellaneous
OtherReaction
4d488e5359293a04a32bace2709761d0f67be5de1412a33fc85af08dc47f7ab7
06e4cfdff0e70e885199cc5de7382cc871277954ed1dd9750edc3ce3b12c44bd
C1CCNCC1
[#8:1]-[C:2](=[O;D1;H0:3])-[C:4]-[C:5]-[NH;D2;+0:6]-[C:7]-[C:8]>>[#8:1]-[C:2](=[O;D1;H0:3])-[C:4]-[C:5]-[N;H0;D3;+0:6](-[C;D1;H3:9])-[C:7]-[C:8]
73
[{"value": 73.0, "product": "CN1C[C@@H](CCC1)C(=O)OCC", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
(R)-Ethyl nipecotate (5.7 g 365 mmol), (prepared by resolution of ethyl nipecotate by treatment with L(+)-tartaric acid as described in J. Org. Chem. 1991, (56), 1168), was dissolved in 38.5% aqueous formaldehyde solution (45 ml) and formic acid (90 ml) and the mixture heated at reflux for 18 hours. The mixture was all...
10.6084/m9.figshare.5104873.v1
null
Secondary amine
Tertiary amine
C1CCNCC1
C1CC[NH]CC1
C1CC[NH]CC1
Other
C=O
null
null
CCOC(=O)[C@@H]1CCCNC1>C=O>CCOC(=O)[C@@H]1CCCN(C)C1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-8a3b45b57fa245f5b86550b96b500be5
CCOC(=O)[C@@H]1CCCN(C)C1>>CN1CCC[C@@H](CO)C1
CN1C[C@@H](CCC1)C(=O)OCC.[H-].[Al+3].[Li+].[H-].[H-].[H-].O.[OH-].[Na+].O>>CN1C[C@@H](CCC1)CO
CCO[C:7]([C@@H:6]1[CH2:5][CH2:4][CH2:3][N:2]([CH3:1])[CH2:9]1)=[O:8]>>[CH3:1][N:2]1[CH2:3][CH2:4][CH2:5][C@@H:6]([CH2:7][OH:8])[CH2:9]1
CCOC(=O)[C@@H]1CCCN(C)C1
CN1CCC[C@@H](CO)C1
null
null
CCOCC.C1CCOC1
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
C1CCNCC1
C-C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[C:3](-[C:4])-[C:5]-[#7:6]>>[#7:6]-[C:5]-[C:3](-[CH2;D2;+0:1]-[OH;D1;+0:2])-[C:4]
94.3
[{"value": 94.0, "product": "CN1C[C@@H](CCC1)CO", "details": "PERCENTYIELD", "is_desired": false}, {"value": 94.3, "product": "CN1C[C@@H](CCC1)CO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
20
CELSIUS
1.5
HOUR
A solution of (R)-ethyl 1-methylpiperidine-3-carboxylate (5.69 g, 33 mmol) in ether (20 ml) was added dropwise to a stirred solution of lithium aluminium hydride (36.6 ml of a 1M solution in THF, 36.6 mmol) in ether (85 ml) cooled to maintain a reaction temperature of 20° C. The mixture was stirred for 1.5 hours at amb...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
C1CC[NH]CC1
HO-
CCOCC.C1CCOC1
20
1.5
CCOC(=O)[C@@H]1CCCN(C)C1>CCOCC.C1CCOC1>CN1CCC[C@@H](CO)C1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-953ee293a6614f7c84aa8f7936ea4c3a
COc1cc2c(Oc3ccc(Cl)cc3F)ncnc2cc1O.c1ccc(P(c2ccccc2)c2ccccc2)cc1>>CN1CCCC(CO)C1.CN1CCC[C@@H](CO)C1
ClC1=CC(=C(OC2=NC=NC3=CC(=C(C=C23)OC)O)C=C1)F.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1>>CN1CC(CCC1)CO.CN1C[C@@H](CCC1)CO
Fc1cc(Cl)ccc1O[c:16]1[n:2][cH:10][n:11][c:14]2[cH:9][c:6]([OH:17])[c:7]([O:8][CH3:1])[cH:18][c:15]21.c1ccc(P(c2cc[cH:12][cH:13]c2)c2cc[cH:3][cH:4][cH:5]2)cc1>>[CH3:1][N:2]1[CH2:3][CH2:4][CH2:5][CH:6]([CH2:7][OH:8])[CH2:9]1.[CH3:10][N:11]1[CH2:12][CH2:13][CH2:14][C@@H:15]([CH2:16][OH:17])[CH2:18]1
COc1cc2c(Oc3ccc(Cl)cc3F)ncnc2cc1O.c1ccc(P(c2ccccc2)c2ccccc2)cc1
CN1CCCC(CO)C1.CN1CCC[C@@H](CO)C1
null
null
ClCCl
Heteroatom Alkylation and Arylation
OtherReaction
b8c593b8a7987448fb9f49e9e1dc564e9d8d35ddf43c6096f8f47b89bcde483e
14ad35e74b335fe2dbf329950ee580105f2b6b3ea5bdb6d5c86b06fec4f8886a
C1CCNCC1.C1CCNCC1
Cl-c1:c:c:c(-O-[c;H0;D3;+0:1]2:[n;H0;D2;+0:2]:[cH;D2;+0:3]:[n;H0;D2;+0:4]:[c;H0;D3;+0:5]3:[cH;D2;+0:6]:[c;H0;D3;+0:7](-[OH;D1;+0:8]):[c;H0;D3;+0:9](-[O;H0;D2;+0:10]-[CH3;D1;+0:11]):[cH;D2;+0:12]:[c;H0;D3;+0:13]:3:2):c(-F):c:1.[cH;D2;+0:14]1:[cH;D2;+0:15]:c:c(-P(-c2:[cH;D2;+0:16]:[cH;D2;+0:17]:[cH;D2;+0:18]:c:c:2)-c2:c:...
null
[]
null
null
30
MINUTE
4-(4-Chloro-2-fluorophenoxy)-7-hydroxy-6-methoxyquinazoline (12.1 g, 38 mmol), (prepared as described for the starting material in Example 5), was suspended in dichloromethane (375 ml) and treated with triphenylphosphine (29.6 g, 113 mmol) then stirred at ambient temperature for 30 minutes. (1-Methylpiperidin-3-yl)meth...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic halide.Ether.Ether.Aromatic alcohol
Primary alcohol.Primary alcohol.Tertiary amine.Tertiary amine
c1ccccc1.c1ccc2ncncc2c1.c1ccccc1.c1ccccc1.c1ccccc1
C1CC[NH]CC1.C1CC[NH]CC1
C1CC[NH]CC1.C1CC[NH]CC1
Other
ClCCl
null
0.5
COc1cc2c(Oc3ccc(Cl)cc3F)ncnc2cc1O.c1ccc(P(c2ccccc2)c2ccccc2)cc1>ClCCl>CN1CCCC(CO)C1.CN1CCC[C@@H](CO)C1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-468c8a1ab0824fd196d274cd310a5cf7
COc1cc2c(Cl)ncnc2cc1OCCCN1CCCC1.Cc1cc2cc(O)ccc2[nH]1>>COc1cc2c(Oc3ccc4[nH]c(C)cc4c3)ncnc2cc1OCCCN1CCCC1
O.ClC1=NC=NC2=CC(=C(C=C12)OC)OCCCN1CCCC1.OC=1C=C2C=C(NC2=CC1)C.C([O-])([O-])=O.[K+].[K+]>>COC=1C=C2C(=NC=NC2=CC1OCCCN1CCCC1)OC=1C=C2C=C(NC2=CC1)C
Cl[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:23]([O:24][CH2:25][CH2:26][CH2:27][N:28]3[CH2:29][CH2:30][CH2:31][CH2:32]3)[cH:22][c:21]2[n:20][cH:19][n:18]1.[OH:7][c:8]1[cH:9][cH:10][c:11]2[nH:12][c:13]([CH3:14])[cH:15][c:16]2[cH:17]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([O:7][c:8]3[cH:9][cH:10][c:11]4[nH:12][c:13]([CH3:14]...
COc1cc2c(Cl)ncnc2cc1OCCCN1CCCC1.Cc1cc2cc(O)ccc2[nH]1
COc1cc2c(Oc3ccc4[nH]c(C)cc4c3)ncnc2cc1OCCCN1CCCC1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
2d25b59c80a437134e7830160726da4e12ee4089c37759035843c1cccd8cd262
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1nc(Oc2ccc3[nH]ccc3c2)c2ccc(OCCCN3CCCC3)cc2n1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[OH;D1;+0:9]-[c:10](:[c:11]):[c:12]>>[c:11]:[c:10](-[O;H0;D2;+0:9]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8]):[c:12]
46.2
[{"value": 46.0, "product": "COC=1C=C2C(=NC=NC2=CC1OCCCN1CCCC1)OC=1C=C2C=C(NC2=CC1)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 46.2, "product": "COC=1C=C2C(=NC=NC2=CC1OCCCN1CCCC1)OC=1C=C2C=C(NC2=CC1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
2
HOUR
A suspension of 4-chloro-6-methoxy-7-(3-(pyrrolidin-1-yl)propoxy)quinazoline (0.13 g, 0.4 mmol), 5-hydroxy-2-methylindole (74 mg, 0.5 mmol) and potassium carbonate (83 mg, 0.6 mmol) in DMF (1.5 ml) was stirred at 100° C. for 2 hours. After cooling to ambient temperature, water (20 ml) was added. The precipitate was col...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2[nH]ccc2c1.c1ccc2ncncc2c1.C1CC[NH]C1
HCl
CN(C)C=O
100
2
COc1cc2c(Cl)ncnc2cc1OCCCN1CCCC1.Cc1cc2cc(O)ccc2[nH]1>CN(C)C=O>COc1cc2c(Oc3ccc4[nH]c(C)cc4c3)ncnc2cc1OCCCN1CCCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e3d1096b942a4a54904d797e6ac7b158
COc1cc(C(=O)O)ccc1O.ClCCCN1CCCC1>>COc1cc(C(=O)O)ccc1OCCCN1CCCC1.Cl
OC1=C(C=C(C(=O)O)C=C1)OC.N1(CCCC1)CCCCl.C([O-])([O-])=O.[K+].[K+].[I-].[K+]>>Cl.COC=1C=C(C(=O)O)C=CC1OCCCN1CCCC1
[CH3:1][O:2][c:3]1[cH:4][c:5]([C:6](=[O:7])[OH:8])[cH:9][cH:10][c:11]1[OH:12].[CH2:13]([CH2:14][CH2:15][N:16]1[CH2:17][CH2:18][CH2:19][CH2:20]1)[Cl:21]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([C:6](=[O:7])[OH:8])[cH:9][cH:10][c:11]1[O:12][CH2:13][CH2:14][CH2:15][N:16]1[CH2:17][CH2:18][CH2:19][CH2:20]1.[ClH:21]
COc1cc(C(=O)O)ccc1O.ClCCCN1CCCC1
COc1cc(C(=O)O)ccc1OCCCN1CCCC1.Cl
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
7e1040116e3a4cf0e8ec5cc7865388d9cd0efabce6d320a1c25a36e411018d8b
d5f4610d46ccc0478471c5bc0fb862644eaf764bbc5d93badb39d54f6ec8e0a5
c1ccc(OCCCN2CCCC2)cc1
[C:1]-[C:2]-[CH2;D2;+0:3]-[Cl;H0;D1;+0:4].[OH;D1;+0:5]-[c:6](:[c:7]):[c:8]>>[C:1]-[C:2]-[CH2;D2;+0:3]-[O;H0;D2;+0:5]-[c:6](:[c:7]):[c:8].[ClH;D0;+0:4]
77.3
[{"value": 77.0, "product": "Cl.COC=1C=C(C(=O)O)C=CC1OCCCN1CCCC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 77.3, "product": "Cl.COC=1C=C(C(=O)O)C=CC1OCCCN1CCCC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
null
null
A mixture of 4-hydroxy-3-methoxybenzoic acid (8.4 g, 50 mmol), 3-(pyrrolidin-1-yl)propyl chloride (14.75 g, 0.1 mol), (J. Am. Chem. Soc. 1955, 77, 2272), potassium carbonate (13.8 g, 0.1 mol) and potassium iodide (1.66 g, 10 mmol) in DMF (150 ml) was stirred and heated at 100° C. for 3 hours. The mixture was allowed to...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic alcohol
Ether
null
null
c1ccccc1.C1CC[NH]C1
null
CN(C)C=O
100
null
COc1cc(C(=O)O)ccc1O.ClCCCN1CCCC1>CN(C)C=O>COc1cc(C(=O)O)ccc1OCCCN1CCCC1.Cl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c78eec71e77643b88860c1c2db4a5eee
COc1cc(C(=O)O)ccc1OCCCN1CCCC1.O=[N+]([O-])O>>COc1cc(C(=O)O)c([N+](=O)[O-])cc1OCCCN1CCCC1
[N+](=O)(O)[O-].Cl.COC=1C=C(C(=O)O)C=CC1OCCCN1CCCC1>>Cl.COC=1C(=CC(=C(C(=O)O)C1)[N+](=O)[O-])OCCCN1CCCC1
[CH3:1][O:2][c:3]1[cH:4][c:5]([C:6](=[O:7])[OH:8])[cH:9][cH:13][c:14]1[O:15][CH2:16][CH2:17][CH2:18][N:19]1[CH2:20][CH2:21][CH2:22][CH2:23]1.O[N+:10](=[O:11])[O-:12]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([C:6](=[O:7])[OH:8])[c:9]([N+:10](=[O:11])[O-:12])[cH:13][c:14]1[O:15][CH2:16][CH2:17][CH2:18][N:19]1[CH2:20][CH2:21][CH2:2...
COc1cc(C(=O)O)ccc1OCCCN1CCCC1.O=[N+]([O-])O
COc1cc(C(=O)O)c([N+](=O)[O-])cc1OCCCN1CCCC1
null
null
C(=O)(C(F)(F)F)O
Functional Group Addition
Aromatic nitration with HNO3
53848b8b2bb4e867226e49db2e60519b24be9379900e3ad7c56af54fe8fde7a5
ddce49825c02b8965f10c8d99e3c841d26e1f136da6037b417c09313e6d73097
c1ccc(OCCCN2CCCC2)cc1
O-[N+;H0;D3:1](-[O;-;D1;H0:2])=[O;D1;H0:3].[O;D1;H0:4]=[C:5](-[O;D1;H1:6])-[c:7](:[c:8]):[cH;D2;+0:9]:[c:10]:[c:11]>>[O;-;D1;H0:2]-[N+;H0;D3:1](=[O;D1;H0:3])-[c;H0;D3;+0:9](:[c:10]:[c:11]):[c:7](-[C:5](=[O;D1;H0:4])-[O;D1;H1:6]):[c:8]
90
[{"value": 90.0, "product": "Cl.COC=1C(=CC(=C(C(=O)O)C1)[N+](=O)[O-])OCCCN1CCCC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 87.9, "product": "Cl.COC=1C(=CC(=C(C(=O)O)C1)[N+](=O)[O-])OCCCN1CCCC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
Fuming nitric acid (2.4 ml, 57.9 mmol) was added slowly at 0° C. to a solution of 3-methoxy-4-(3-(pyrrolidin-1-yl)propoxy)benzoic acid hydrochloride (12.15 g, 38.17 mmol) in TFA (40 ml). The cooling bath was removed and the reaction mixture stirred at ambient temperature for 1 hour. The TFA was removed by evaporation a...
10.6084/m9.figshare.5104873.v1
null
Nitrate
Nitro group
c1ccccc1
c1ccccc1
c1ccccc1.C1CC[NH]C1
HO-
C(=O)(C(F)(F)F)O
null
1
COc1cc(C(=O)O)ccc1OCCCN1CCCC1.O=[N+]([O-])O>C(=O)(C(F)(F)F)O>COc1cc(C(=O)O)c([N+](=O)[O-])cc1OCCCN1CCCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-9f93506979e14002b2e5ba7689e3e458
COc1cc(C(=O)O)c([N+](=O)[O-])cc1OCCCN1CCCC1>>COc1cc(C(N)=O)c([N+](=O)[O-])cc1OCCCN1CCCC1
Cl.COC=1C(=CC(=C(C(=O)O)C1)[N+](=O)[O-])OCCCN1CCCC1.CN(C)C=O>>COC=1C(=CC(=C(C(=O)N)C1)[N+](=O)[O-])OCCCN1CCCC1
O[C:6]([c:5]1[cH:4][c:3]([O:2][CH3:1])[c:14]([O:15][CH2:16][CH2:17][CH2:18][N:19]2[CH2:20][CH2:21][CH2:22][CH2:23]2)[cH:13][c:9]1[N+:10](=[O:11])[O-:12])=[O:8]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([C:6]([NH2:7])=[O:8])[c:9]([N+:10](=[O:11])[O-:12])[cH:13][c:14]1[O:15][CH2:16][CH2:17][CH2:18][N:19]1[CH2:20][CH2:21][CH2:22][CH...
COc1cc(C(=O)O)c([N+](=O)[O-])cc1OCCCN1CCCC1
COc1cc(C(N)=O)c([N+](=O)[O-])cc1OCCCN1CCCC1
null
null
S(=O)(Cl)Cl
Functional Group Interconversion
OtherReaction
e1b1a1f71ee10336b9e90a021457b106dbfe08a22161aaad6804675a8134a46f
5d384be3554a01fd49be5eb779c3b10075a4cc9a2373eb20aaa867286d4e28a9
c1ccc(OCCCN2CCCC2)cc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]>>[N;D1;H2:6]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
73
[{"value": 73.0, "product": "COC=1C(=CC(=C(C(=O)N)C1)[N+](=O)[O-])OCCCN1CCCC1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
1.5
HOUR
A solution of 5-methoxy-2-nitro-4-(3-(pyrrolidin-1-yl)propoxy)benzoic acid hydrochloride (9.63 g, 24 mmol) in thionyl chloride (20 ml) and DMF (50 μl) was heated at 45° C. for 1.5 hours. The excess thionyl chloride was removed by evaporation and by azeotroping with toluene (×2). The resulting solid was suspended in THF...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Primary amide
null
null
c1ccccc1.C1CC[NH]C1
null
S(=O)(Cl)Cl
null
1.5
COc1cc(C(=O)O)c([N+](=O)[O-])cc1OCCCN1CCCC1>S(=O)(Cl)Cl>COc1cc(C(N)=O)c([N+](=O)[O-])cc1OCCCN1CCCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-65c85e4819d640f5a613400a453478e4
COc1cc(C(N)=O)c([N+](=O)[O-])cc1OCCCN1CCCC1>>COc1cc(C(N)=O)c(N)cc1OCCCN1CCCC1
Cl.COC=1C(=CC(=C(C(=O)N)C1)[N+](=O)[O-])OCCCN1CCCC1>>Cl.NC1=C(C(=O)N)C=C(C(=C1)OCCCN1CCCC1)OC
O=[N+:10]([O-])[c:9]1[c:5]([C:6]([NH2:7])=[O:8])[cH:4][c:3]([O:2][CH3:1])[c:12]([O:13][CH2:14][CH2:15][CH2:16][N:17]2[CH2:18][CH2:19][CH2:20][CH2:21]2)[cH:11]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]([C:6]([NH2:7])=[O:8])[c:9]([NH2:10])[cH:11][c:12]1[O:13][CH2:14][CH2:15][CH2:16][N:17]1[CH2:18][CH2:19][CH2:20][CH2:21]1
COc1cc(C(N)=O)c([N+](=O)[O-])cc1OCCCN1CCCC1
COc1cc(C(N)=O)c(N)cc1OCCCN1CCCC1
null
[Fe]
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc(OCCCN2CCCC2)cc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]-[C:5](-[N;D1;H2:6])=[O;D1;H0:7]>>[N;D1;H2:6]-[C:5](=[O;D1;H0:7])-[c:4]:[c:2](-[NH2;D1;+0:1]):[c:3]
85
[{"value": 85.0, "product": "Cl.NC1=C(C(=O)N)C=C(C(=C1)OCCCN1CCCC1)OC", "details": "PERCENTYIELD", "is_desired": false}]
50
CELSIUS
null
null
Concentrated hydrochloric acid (5 ml) was added to a suspension of 5-methoxy-2-nitro-4-(3-(pyrrolidin-1-yl)propoxy)benzamide (1.5 g, 4.64 mmol) in methanol (20 ml) and the mixture was heated at 50° C. to give a solution. Iron powder (1.3 g, 23.2 mmol) was added in portions and the reaction mixture was then heated at re...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1.C1CC[NH]C1
Other
[Fe].CO
50
null
COc1cc(C(N)=O)c([N+](=O)[O-])cc1OCCCN1CCCC1>[Fe].CO>COc1cc(C(N)=O)c(N)cc1OCCCN1CCCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e8213d2577f9480c993b2fc592165aac
COc1cc(C(N)=O)c(N)cc1OCCCN1CCCC1>>COc1cc2c(O)ncnc2cc1OCCCN1CCCC1
Cl.NC1=C(C(=O)N)C=C(C(=C1)OCCCN1CCCC1)OC.CN(C)C=NC=[N+](C)C.[Cl-].C(C)(=O)O.C(C)(=O)[O-].[Na+]>>OC1=NC=NC2=CC(=C(C=C12)OC)OCCCN1CCCC1
[CH3:1][O:2][c:3]1[cH:4][c:5]([C:6](=[O:7])[NH2:8])[c:11]([NH2:10])[cH:12][c:13]1[O:14][CH2:15][CH2:16][CH2:17][N:18]1[CH2:19][CH2:20][CH2:21][CH2:22]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([OH:7])[n:8][cH:9][n:10][c:11]2[cH:12][c:13]1[O:14][CH2:15][CH2:16][CH2:17][N:18]1[CH2:19][CH2:20][CH2:21][CH2:22]1
COc1cc(C(N)=O)c(N)cc1OCCCN1CCCC1
COc1cc2c(O)ncnc2cc1OCCCN1CCCC1
null
null
O1CCOCC1
Aromatic Heterocycle Formation
OtherReaction
0a83a7d1eeda533da1fe0ab49b40addde9a79d36d3b4681a7c25cbc84aae3632
c7f1baf6d039a31bf559cfdf0b5118c8ff66e7eb348eec43bb09814b0890990b
c1ncc2ccc(OCCCN3CCCC3)cc2n1
[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4](-[C;H0;D3;+0:5](-[NH2;D1;+0:6])=[O;H0;D1;+0:7]):[c:8]>>[OH;D1;+0:7]-[c;H0;D3;+0:5]1:[n;H0;D2;+0:6]:[c:9]:[n;H0;D2;+0:1]:[c:2](:[c:3]):[c:4]:1:[c:8]
92.6
[{"value": 83.0, "product": "OC1=NC=NC2=CC(=C(C=C12)OC)OCCCN1CCCC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 92.6, "product": "OC1=NC=NC2=CC(=C(C=C12)OC)OCCCN1CCCC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 2-amino-5-methoxy-4-(3-(pyrrolidin-1-yl)propoxy)benzamide hydrochloride (5.92 g, 16.2 mmol) and Gold's reagent (3.5 g, 21.4 mmol) in dioxane (50 ml) was heated at reflux for 5 hours. Acetic acid (0.7 ml) and sodium acetate (1.33 g) were added to the reaction mixture which was heated at reflux for a further...
10.6084/m9.figshare.5104873.v1
null
Primary amide.Primary amine
Aromatic alcohol
c1ccccc1
c1ccc2ncncc2c1
c1ccc2ncncc2c1.C1CC[NH]C1
Other
O1CCOCC1
null
null
COc1cc(C(N)=O)c(N)cc1OCCCN1CCCC1>O1CCOCC1>COc1cc2c(O)ncnc2cc1OCCCN1CCCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f0abda1a6a304b70a4c0bcb58c3af872
COc1cc2c(O)ncnc2cc1OCCCN1CCCC1.O=S(Cl)Cl>>COc1cc2c(Cl)ncnc2cc1OCCCN1CCCC1
OC1=NC=NC2=CC(=C(C=C12)OC)OCCCN1CCCC1.S(=O)(Cl)Cl>>ClC1=NC=NC2=CC(=C(C=C12)OC)OCCCN1CCCC1
O[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:13]([O:14][CH2:15][CH2:16][CH2:17][N:18]3[CH2:19][CH2:20][CH2:21][CH2:22]3)[cH:12][c:11]2[n:10][cH:9][n:8]1.O=S(Cl)[Cl:7]>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([Cl:7])[n:8][cH:9][n:10][c:11]2[cH:12][c:13]1[O:14][CH2:15][CH2:16][CH2:17][N:18]1[CH2:19][CH2:20][CH2:21][CH2:22]1
COc1cc2c(O)ncnc2cc1OCCCN1CCCC1.O=S(Cl)Cl
COc1cc2c(Cl)ncnc2cc1OCCCN1CCCC1
null
null
CN(C)C=O
Functional Group Interconversion
Alcohol to chloride_SOCl2
b0b0f8b7642d018e3b261231985ddd65d16d4d42cce7aa11791e49c826337b90
e71580a8ffadb7b2717ecd7d68c1d3c0ca161ba5e6a787a49dad5a1359adc993
c1ncc2ccc(OCCCN3CCCC3)cc2n1
Cl-S(=O)-[Cl;H0;D1;+0:1].O-[c;H0;D3;+0:2]1:[#7;a:3]:[c:4]:[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9]>>[Cl;H0;D1;+0:1]-[c;H0;D3;+0:2]1:[#7;a:3]:[c:4]:[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9]
null
[]
null
null
null
null
A mixture of 4-hydroxy-6-methoxy-7-(3-(pyrrolidin-1-yl)propoxy)quinazoline (1.7 g, 5 mmol) and thionyl chloride (25 ml) containing DMF (0.2 ml) was heated at reflux for 3 hours. Excess thionyl chloride was removed by evaporation and by azeotroping with toluene (×2). The residue was suspended in ether and 10% aqueous so...
10.6084/m9.figshare.5104873.v1
null
Aromatic alcohol
Aromatic halide
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2ncncc2c1.C1CC[NH]C1
HCl
CN(C)C=O
null
null
COc1cc2c(O)ncnc2cc1OCCCN1CCCC1.O=S(Cl)Cl>CN(C)C=O>COc1cc2c(Cl)ncnc2cc1OCCCN1CCCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-86f4f72f75ec49408153ebc85b29e367
CC(C)(C)OC(=O)N1CCC(CO)CC1.Cc1ccccc1S(=O)(=O)Cl>>Cc1ccc(S(=O)(=O)OCC2CCN(C(=O)OC(C)(C)C)CC2)cc1
C=1(C(=CC=CC1)S(=O)(=O)Cl)C.OCC1CCN(CC1)C(=O)OC(C)(C)C.N12CCN(CC1)CC2>>CC1=CC=C(C=C1)S(=O)(=O)OCC1CCN(CC1)C(=O)OC(C)(C)C
[OH:9][CH2:10][CH:11]1[CH2:12][CH2:13][N:14]([C:15](=[O:16])[O:17][C:18]([CH3:19])([CH3:20])[CH3:21])[CH2:22][CH2:23]1.Cl[S:6]([c:5]1[c:2]([CH3:1])[cH:3][cH:4][cH:25][cH:24]1)(=[O:7])=[O:8]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([S:6](=[O:7])(=[O:8])[O:9][CH2:10][CH:11]2[CH2:12][CH2:13][N:14]([C:15](=[O:16])[O:17][C:18]([CH3:...
CC(C)(C)OC(=O)N1CCC(CO)CC1.Cc1ccccc1S(=O)(=O)Cl
Cc1ccc(S(=O)(=O)OCC2CCN(C(=O)OC(C)(C)C)CC2)cc1
null
null
CCOCC.COC(C)(C)C
Acylation
OtherReaction
6dd26378b7c569e7e73da2c430efcb9bc58014e30edce94cf052e575133a80c4
436a9e21ae4d378d7049998650bf5bf959f4c8094cc386d78e7e073ba98e619a
O=S(=O)(OCC1CCNCC1)c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c;H0;D3;+0:4]1:[c:5]:[cH;D2;+0:6]:[cH;D2;+0:7]:[c:8]:[c;H0;D3;+0:9]:1-[C;D1;H3:10].[C:11]-[C:12]-[OH;D1;+0:13]>>[C:11]-[C:12]-[O;H0;D2;+0:13]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c;H0;D3;+0:4]1:[c:5]:[cH;D2;+0:6]:[c;H0;D3;+0:9](-[C;D1;H3:10]):[c:8]:[cH;D2;+0:7]:1
62,906.5
[{"value": 85.0, "product": "CC1=CC=C(C=C1)S(=O)(=O)OCC1CCN(CC1)C(=O)OC(C)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 62906.5, "product": "CC1=CC=C(C=C1)S(=O)(=O)OCC1CCN(CC1)C(=O)OC(C)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
To a solution of 4-hydroxymethyl-1-tert-butyloxycarbonylpiperidine (52.5 g, 0.244 mol) in tert-butyl methyl ether (525 ml) was added 1,4-diazabicyclo[2.2.2]octane (42.4 g, 0.378 mol). After stirring for 15 minutes at ambient temperature, the mixture was cooled to 5° C. and a solution of toluene sulphonyl chloride (62.8...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Sulfonyl halide
Tosylate
c1ccccc1
c1ccccc1
c1ccccc1.C1CC[NH]CC1
HCl
CCOCC.COC(C)(C)C
null
0.25
CC(C)(C)OC(=O)N1CCC(CO)CC1.Cc1ccccc1S(=O)(=O)Cl>CCOCC.COC(C)(C)C>Cc1ccc(S(=O)(=O)OCC2CCN(C(=O)OC(C)(C)C)CC2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-fd0a40d6fd0f4a0fa3e2bcf016c3a5a1
CCOC(=O)c1ccc(O)c(OC)c1.Cc1ccc(S(=O)(=O)OCC2CCN(C(=O)OC(C)(C)C)CC2)cc1>>CCOC(=O)c1ccc(OCC2CCN(C(=O)OC(C)(C)C)CC2)c(OC)c1
COC=1C=C(C(=O)OCC)C=CC1O.C([O-])([O-])=O.[K+].[K+].CC1=CC=C(C=C1)S(=O)(=O)OCC1CCN(CC1)C(=O)OC(C)(C)C>>COC=1C=C(C(=O)OCC)C=CC1OCC1CCN(CC1)C(=O)OC(C)(C)C
[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][c:9]([OH:10])[c:25]([O:26][CH3:27])[cH:28]1.Cc1ccc(S(=O)(=O)O[CH2:11][CH:12]2[CH2:13][CH2:14][N:15]([C:16](=[O:17])[O:18][C:19]([CH3:20])([CH3:21])[CH3:22])[CH2:23][CH2:24]2)cc1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][c:9]([O:10][CH2:11][CH:12]2[CH2:13][CH2...
CCOC(=O)c1ccc(O)c(OC)c1.Cc1ccc(S(=O)(=O)OCC2CCN(C(=O)OC(C)(C)C)CC2)cc1
CCOC(=O)c1ccc(OCC2CCN(C(=O)OC(C)(C)C)CC2)c(OC)c1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
OtherReaction
b5213736859cf91483a02f350869986d9b7674724716adef8a5d7a4bbdb79574
3d107e624e135e10014c7bf413dd0be27e1e4488f039e545b94cb1680b764158
c1ccc(OCC2CCNCC2)cc1
C-c1:c:c:c(-S(=O)(=O)-O-[CH2;D2;+0:1]-[C:2](-[C:3])-[C:4]):c:c:1.[OH;D1;+0:5]-[c:6](:[c:7]):[c:8]>>[C:3]-[C:2](-[CH2;D2;+0:1]-[O;H0;D2;+0:5]-[c:6](:[c:7]):[c:8])-[C:4]
89
[{"value": 89.0, "product": "COC=1C=C(C(=O)OCC)C=CC1OCC1CCN(CC1)C(=O)OC(C)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 89.0, "product": "COC=1C=C(C(=O)OCC)C=CC1OCC1CCN(CC1)C(=O)OC(C)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
95
CELSIUS
2.5
HOUR
To a suspension of ethyl 3-methoxy-4-hydroxybenzoate (19.6 g, 0.1 mol) and potassium carbonate (28 g, 0.2 mol) in dry DMF (200 ml) was added 4-(4-methylphenylsulphonyloxymethyl)-1-tert-butyloxycarbonylpiperidine (40 g, 0.11 mol). After stirring at 95° C. for 2.5 hours, the mixture was cooled to ambient temperature and ...
10.6084/m9.figshare.5104873.v1
null
Tosylate.Aromatic alcohol
Ether
c1ccccc1
null
c1ccccc1.C1CC[NH]CC1
TsOH.HO-
CN(C)C=O
95
2.5
CCOC(=O)c1ccc(O)c(OC)c1.Cc1ccc(S(=O)(=O)OCC2CCN(C(=O)OC(C)(C)C)CC2)cc1>CN(C)C=O>CCOC(=O)c1ccc(OCC2CCN(C(=O)OC(C)(C)C)CC2)c(OC)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0d70b38b1805414687e476e36009fc18
CCOC(=O)c1ccc(OCC2CCN(C(=O)OC(C)(C)C)CC2)c(OC)c1>>CCOC(=O)c1ccc(OCC2CCN(C)CC2)c(OC)c1
Cl.CCOCC.COC=1C=C(C(=O)OCC)C=CC1OCC1CCN(CC1)C(=O)OC(C)(C)C.C=O>>COC=1C=C(C(=O)OCC)C=CC1OCC1CCN(CC1)C
CC(C)(C)O[C:16](=O)[N:15]1[CH2:14][CH2:13][CH:12]([CH2:11][O:10][c:9]2[cH:8][cH:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[cH:22][c:19]2[O:20][CH3:21])[CH2:18][CH2:17]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][cH:8][c:9]([O:10][CH2:11][CH:12]2[CH2:13][CH2:14][N:15]([CH3:16])[CH2:17][CH2:18]2)[c:19]([O:20][CH3:21])[...
CCOC(=O)c1ccc(OCC2CCN(C(=O)OC(C)(C)C)CC2)c(OC)c1
CCOC(=O)c1ccc(OCC2CCN(C)CC2)c(OC)c1
null
null
C(=O)O
Reduction
OtherReaction
dcda46d15ef9f01c1f93228fbde5fe507f031b166ebcdcda0b018d3445dde9e4
414023a339cb5e5ca20834c6434c67bcea724431433bac28293e7fcfb67a2a9e
c1ccc(OCC2CCNCC2)cc1
C-C(-C)(-C)-O-[C;H0;D3;+0:1](=O)-[#7:2](-[C:3])-[C:4]>>[C:3]-[#7:2](-[CH3;D1;+0:1])-[C:4]
111.9
[{"value": 111.9, "product": "COC=1C=C(C(=O)OCC)C=CC1OCC1CCN(CC1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
95
CELSIUS
3
HOUR
To a solution of ethyl 3-methoxy-4-(1-tert-butyloxycarbonylpiperidin-4-ylmethoxy)benzoate (35 g, 89 mmol) in formic acid (35 ml) was added formaldehyde (12M, 37% in water, 35 ml, 420 mmol). After stirring at 95° C. for 3 hours, the volatiles were removed by evaporation. The residue was dissolved in methylene chloride a...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
null
null
null
c1ccccc1.C1CC[NH]CC1
HO-
C(=O)O
95
3
CCOC(=O)c1ccc(OCC2CCN(C(=O)OC(C)(C)C)CC2)c(OC)c1>C(=O)O>CCOC(=O)c1ccc(OCC2CCN(C)CC2)c(OC)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5db72145fc924655aa52ca487a293c36
CCOC(=O)c1ccc(OCC2CCN(C)CC2)c(OC)c1.O=[N+]([O-])O>>CCOC(=O)c1cc(OC)c(OCC2CCN(C)CC2)cc1[N+](=O)[O-]
COC=1C=C(C(=O)OCC)C=CC1OCC1CCN(CC1)C.C(=O)(C(F)(F)F)O.[N+](=O)(O)[O-]>>COC=1C=C(C(=O)OCC)C(=CC1OCC1CCN(CC1)C)[N+](=O)[O-]
[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][c:8]([O:9][CH3:10])[c:11]([O:12][CH2:13][CH:14]2[CH2:15][CH2:16][N:17]([CH3:18])[CH2:19][CH2:20]2)[cH:21][cH:22]1.O[N+:23](=[O:24])[O-:25]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][c:8]([O:9][CH3:10])[c:11]([O:12][CH2:13][CH:14]2[CH2:15][CH2:16][N:17]([CH3:18])[CH2:19][C...
CCOC(=O)c1ccc(OCC2CCN(C)CC2)c(OC)c1.O=[N+]([O-])O
CCOC(=O)c1cc(OC)c(OCC2CCN(C)CC2)cc1[N+](=O)[O-]
null
null
C(Cl)Cl
Functional Group Addition
Aromatic nitration with HNO3
53848b8b2bb4e867226e49db2e60519b24be9379900e3ad7c56af54fe8fde7a5
ddce49825c02b8965f10c8d99e3c841d26e1f136da6037b417c09313e6d73097
c1ccc(OCC2CCNCC2)cc1
O-[N+;H0;D3:1](-[O;-;D1;H0:2])=[O;D1;H0:3].[C:4]-[#8:5]-[C:6](=[O;D1;H0:7])-[c:8](:[c:9]):[cH;D2;+0:10]:[c:11]:[c:12]>>[C:4]-[#8:5]-[C:6](=[O;D1;H0:7])-[c:8](:[c:9]):[c;H0;D3;+0:10](-[N+;H0;D3:1](-[O;-;D1;H0:2])=[O;D1;H0:3]):[c:11]:[c:12]
90.6
[{"value": 82.0, "product": "COC=1C=C(C(=O)OCC)C(=CC1OCC1CCN(CC1)C)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 90.6, "product": "COC=1C=C(C(=O)OCC)C(=CC1OCC1CCN(CC1)C)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
A solution of ethyl 3-methoxy-4-(1-methylpiperidin-4-ylmethoxy)benzoate (30.6 g, 89 mmol) in methylene chloride (75 ml) was cooled to 0–5° C. TFA (37.5 ml) was added followed by the dropwise addition over 15 minutes of a solution of fuming 24M nitric acid (7.42 ml, 178 mmol) in methylene chloride (15 ml). After complet...
10.6084/m9.figshare.5104873.v1
null
Nitrate
Nitro group
c1ccccc1
c1ccccc1
c1ccccc1.C1CC[NH]CC1
HO-
C(Cl)Cl
null
2
CCOC(=O)c1ccc(OCC2CCN(C)CC2)c(OC)c1.O=[N+]([O-])O>C(Cl)Cl>CCOC(=O)c1cc(OC)c(OCC2CCN(C)CC2)cc1[N+](=O)[O-]
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d82fc98a94e14acc8e1f82ee567bacfc
CCOC(=O)c1cc(OC)c(OCC2CCN(C)CC2)cc1[N+](=O)[O-]>>CCOC(=O)c1cc(OC)c(OCC2CCN(C)CC2)cc1N
COC=1C=C(C(=O)OCC)C(=CC1OCC1CCN(CC1)C)[N+](=O)[O-].[H][H]>>NC1=CC(=C(C=C1C(=O)OCC)OC)OCC1CCN(CC1)C
O=[N+:23]([O-])[c:22]1[c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[cH:7][c:8]([O:9][CH3:10])[c:11]([O:12][CH2:13][CH:14]2[CH2:15][CH2:16][N:17]([CH3:18])[CH2:19][CH2:20]2)[cH:21]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][c:8]([O:9][CH3:10])[c:11]([O:12][CH2:13][CH:14]2[CH2:15][CH2:16][N:17]([CH3:18])[CH2:19][CH2:20]2)[...
CCOC(=O)c1cc(OC)c(OCC2CCN(C)CC2)cc1[N+](=O)[O-]
CCOC(=O)c1cc(OC)c(OCC2CCN(C)CC2)cc1N
null
[Pt]
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc(OCC2CCNCC2)cc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]-[C:5](-[#8:6])=[O;D1;H0:7]>>[#8:6]-[C:5](=[O;D1;H0:7])-[c:4]:[c:2](-[NH2;D1;+0:1]):[c:3]
80
[{"value": 80.0, "product": "NC1=CC(=C(C=C1C(=O)OCC)OC)OCC1CCN(CC1)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 80.0, "product": "NC1=CC(=C(C=C1C(=O)OCC)OC)OCC1CCN(CC1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A suspension of ethyl 3-methoxy-4-(1-methylpiperidin-4-ylmethoxy)-6-nitrobenzoate (3.89 g, 10 mmol) in methanol (80 ml) containing 10% platinum on activated carbon (50% wet) (389 mg) was hydrogenated at 1.8 atmospheres pressure until uptake of hydrogen ceased. The mixture was filtered and the filtrate was evaporated. T...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1.C1CC[NH]CC1
Other
[Pt].CO
null
null
CCOC(=O)c1cc(OC)c(OCC2CCN(C)CC2)cc1[N+](=O)[O-]>[Pt].CO>CCOC(=O)c1cc(OC)c(OCC2CCN(C)CC2)cc1N
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-1e7f1c8f0d364e399633d11e965d2672
CCOC(=O)c1cc(OC)c(OCC2CCN(C)CC2)cc1N.N=CN>>COc1cc2c(=O)[nH]cnc2cc1OCC1CCN(C)CC1
C(C)(=O)O.C(=N)N.NC1=CC(=C(C=C1C(=O)OCC)OC)OCC1CCN(CC1)C.C(C)(=O)O.C(=N)N>>COC=1C=C2C(NC=NC2=CC1OCC1CCN(CC1)C)=O
CCO[C:6]([c:5]1[cH:4][c:3]([O:2][CH3:1])[c:13]([O:14][CH2:15][CH:16]2[CH2:17][CH2:18][N:19]([CH3:20])[CH2:21][CH2:22]2)[cH:12][c:11]1[NH2:10])=[O:7].N[CH:9]=[NH:8]>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6](=[O:7])[nH:8][cH:9][n:10][c:11]2[cH:12][c:13]1[O:14][CH2:15][CH:16]1[CH2:17][CH2:18][N:19]([CH3:20])[CH2:21][CH2:22]1
CCOC(=O)c1cc(OC)c(OCC2CCN(C)CC2)cc1N.N=CN
COc1cc2c(=O)[nH]cnc2cc1OCC1CCN(C)CC1
null
null
COCCO
Aromatic Heterocycle Formation
OtherReaction
13c011143e351c3bbcd763cf1f04e086fd7ad2457d617cac850e1edc36b71aac
36efa24579e0043fdba8918e78f1d75cb4504837c08d344d01203f5fa64bfaef
O=c1[nH]cnc2cc(OCC3CCNCC3)ccc12
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5](-[NH2;D1;+0:6]):[c:7].N-[CH;D2;+0:8]=[NH;D1;+0:9]>>[O;D1;H0:2]=[c;H0;D3;+0:1]1:[nH;D2;+0:9]:[cH;D2;+0:8]:[n;H0;D2;+0:6]:[c:5](:[c:7]):[c:3]:1:[c:4]
83.7
[{"value": 70.0, "product": "COC=1C=C2C(NC=NC2=CC1OCC1CCN(CC1)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 83.7, "product": "COC=1C=C2C(NC=NC2=CC1OCC1CCN(CC1)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
115
CELSIUS
30
MINUTE
A solution of ethyl 6-amino-3-methoxy-4-(1-methylpiperidin-4-ylmethoxy)benzoate (16.1 g, 50 mmol) in 2-methoxyethanol (160 ml) containing formamidine acetate (5.2 g, 50 mmol) was heated at 115° C. for 2 hours. Formamidine acetate (10.4 g, 100 mmol) was added in portions every 30 minutes during 4 hours. Heating was prol...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine.Primary amine
null
c1ccccc1
c1ccc2ncncc2c1
c1ccc2ncncc2c1.C1CC[NH]CC1
HO-
COCCO
115
0.5
CCOC(=O)c1cc(OC)c(OCC2CCN(C)CC2)cc1N.N=CN>COCCO>COc1cc2c(=O)[nH]cnc2cc1OCC1CCN(C)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-2a8ee02ecab44445b12b1c97515591ac
COc1cc2c(=O)[nH]cnc2cc1OCC1CCN(C)CC1.O=S(Cl)Cl>>COc1cc2c(Cl)ncnc2cc1OCC1CCN(C)CC1
COC=1C=C2C(NC=NC2=CC1OCC1CCN(CC1)C)=O.CN(C)C=O.S(=O)(Cl)Cl>>ClC1=NC=NC2=CC(=C(C=C12)OC)OCC1CCN(CC1)C
O=[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:13]([O:14][CH2:15][CH:16]3[CH2:17][CH2:18][N:19]([CH3:20])[CH2:21][CH2:22]3)[cH:12][c:11]2[n:10][cH:9][nH:8]1.O=S(Cl)[Cl:7]>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([Cl:7])[n:8][cH:9][n:10][c:11]2[cH:12][c:13]1[O:14][CH2:15][CH:16]1[CH2:17][CH2:18][N:19]([CH3:20])[CH2:21][CH2:22]1
COc1cc2c(=O)[nH]cnc2cc1OCC1CCN(C)CC1.O=S(Cl)Cl
COc1cc2c(Cl)ncnc2cc1OCC1CCN(C)CC1
null
null
null
Functional Group Interconversion
OtherReaction
3788560e87eee8765e749543914a91a512631307b97fad163ebef894d2a0ea68
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1ncc2ccc(OCC3CCNCC3)cc2n1
Cl-S(=O)-[Cl;H0;D1;+0:1].O=[c;H0;D3;+0:2]1:[nH;D2;+0:3]:[c:4]:[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9]>>[Cl;H0;D1;+0:1]-[c;H0;D3;+0:2]1:[n;H0;D2;+0:3]:[c:4]:[#7;a:5]:[c:6](:[c:7]):[c:8]:1:[c:9]
98
[{"value": 98.0, "product": "ClC1=NC=NC2=CC(=C(C=C12)OC)OCC1CCN(CC1)C", "details": "PERCENTYIELD", "is_desired": false}]
85
CELSIUS
null
null
A solution of 6-methoxy-7-((1-methylpiperidin-4-yl)methoxy)-3,4-dihydroquinazolin-4-one (2.8 g, 9.24 mmol) in thionyl chloride (28 ml) containing DMF (2801 μl) was refluxed at 85° C. for 1 hour. After cooling, the volatiles were removed by evaporation. The precipitate was triturated with ether, filtered, washed with et...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2ncncc2c1.C1CC[NH]CC1
HCl
null
85
null
COc1cc2c(=O)[nH]cnc2cc1OCC1CCN(C)CC1.O=S(Cl)Cl>>COc1cc2c(Cl)ncnc2cc1OCC1CCN(C)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c6abee09358844058b596e6adcde4f1a
COc1cc2c(Cl)ncnc2cc1OCC1CCN(C)CC1.Cc1cc2cc(O)ccc2[nH]1>>COc1cc2c(Oc3ccc4[nH]c(C)cc4c3)ncnc2cc1OCC1CCN(C)CC1
ClC1=NC=NC2=CC(=C(C=C12)OC)OCC1CCN(CC1)C.OC=1C=C2C=C(NC2=CC1)C>>COC=1C=C2C(=NC=NC2=CC1OCC1CCN(CC1)C)OC=1C=C2C=C(NC2=CC1)C
Cl[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:23]([O:24][CH2:25][CH:26]3[CH2:27][CH2:28][N:29]([CH3:30])[CH2:31][CH2:32]3)[cH:22][c:21]2[n:20][cH:19][n:18]1.[OH:7][c:8]1[cH:9][cH:10][c:11]2[nH:12][c:13]([CH3:14])[cH:15][c:16]2[cH:17]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([O:7][c:8]3[cH:9][cH:10][c:11]4[nH:12][c:13]([CH3:14...
COc1cc2c(Cl)ncnc2cc1OCC1CCN(C)CC1.Cc1cc2cc(O)ccc2[nH]1
COc1cc2c(Oc3ccc4[nH]c(C)cc4c3)ncnc2cc1OCC1CCN(C)CC1
null
null
null
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
2d25b59c80a437134e7830160726da4e12ee4089c37759035843c1cccd8cd262
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1nc(Oc2ccc3[nH]ccc3c2)c2ccc(OCC3CCNCC3)cc2n1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[OH;D1;+0:9]-[c:10](:[c:11]):[c:12]>>[c:11]:[c:10](-[O;H0;D2;+0:9]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8]):[c:12]
79.2
[{"value": 79.0, "product": "COC=1C=C2C(=NC=NC2=CC1OCC1CCN(CC1)C)OC=1C=C2C=C(NC2=CC1)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 79.2, "product": "COC=1C=C2C(=NC=NC2=CC1OCC1CCN(CC1)C)OC=1C=C2C=C(NC2=CC1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Using a procedure analogous to that described for Example 9, 4-chloro-6-methoxy-7-((1-methylpiperidin-4-yl)methoxy)quinazoline (0.13 g, 0.4 mmol), (prepared as described for the starting material in Example 10), was reacted with 5-hydroxy-2-methylindole (74 mg, 0.5 mol) to give 6-methoxy-4-(2-methylindol-5-yloxy)-7-((1...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2[nH]ccc2c1.c1ccc2ncncc2c1.C1CC[NH]CC1
HCl
null
null
null
COc1cc2c(Cl)ncnc2cc1OCC1CCN(C)CC1.Cc1cc2cc(O)ccc2[nH]1>>COc1cc2c(Oc3ccc4[nH]c(C)cc4c3)ncnc2cc1OCC1CCN(C)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e69b470660054ac7b140a6bbb2387121
COc1cc2c(Cl)ncnc2cc1OCC1CCN(CCS(C)(=O)=O)CC1.Oc1ccc2cccnc2c1>>COc1cc2c(Oc3ccc4cccnc4c3)ncnc2cc1OCC1CCN(CCS(C)(=O)=O)CC1
ClC1=NC=NC2=CC(=C(C=C12)OC)OCC1CCN(CC1)CCS(=O)(=O)C.OC1=CC=C2C=CC=NC2=C1.C([O-])([O-])=O.[K+].[K+]>>COC=1C=C2C(=NC=NC2=CC1OCC1CCN(CC1)CCS(=O)(=O)C)OC1=CC=C2C=CC=NC2=C1
Cl[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:23]([O:24][CH2:25][CH:26]3[CH2:27][CH2:28][N:29]([CH2:30][CH2:31][S:32]([CH3:33])(=[O:34])=[O:35])[CH2:36][CH2:37]3)[cH:22][c:21]2[n:20][cH:19][n:18]1.[OH:7][c:8]1[cH:9][cH:10][c:11]2[cH:12][cH:13][cH:14][n:15][c:16]2[cH:17]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([O:7][c:8]3[cH:...
COc1cc2c(Cl)ncnc2cc1OCC1CCN(CCS(C)(=O)=O)CC1.Oc1ccc2cccnc2c1
COc1cc2c(Oc3ccc4cccnc4c3)ncnc2cc1OCC1CCN(CCS(C)(=O)=O)CC1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
2d25b59c80a437134e7830160726da4e12ee4089c37759035843c1cccd8cd262
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1cnc2cc(Oc3ncnc4cc(OCC5CCNCC5)ccc34)ccc2c1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[#7;a:9]:[c:10]:[c:11]:[c:12](-[OH;D1;+0:13]):[c:14]>>[#7;a:9]:[c:10]:[c:11]:[c:12](-[O;H0;D2;+0:13]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8]):[c:14]
76
[{"value": 76.0, "product": "COC=1C=C2C(=NC=NC2=CC1OCC1CCN(CC1)CCS(=O)(=O)C)OC1=CC=C2C=CC=NC2=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 75.2, "product": "COC=1C=C2C(=NC=NC2=CC1OCC1CCN(CC1)CCS(=O)(=O)C)OC1=CC=C2C=CC=NC2=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
2
HOUR
To a solution of 4-chloro-6-methoxy-7-((1-(2-methylsulphonylethyl)piperidin-4-yl)methoxy)quinazoline (115 mg, 0.28 mmol) and 7-hydroxyquinoline (50 mg, 0.33 mmol) in DMF (1.5 ml) was added potassium carbonate (60 mg, 0.42 mmol). The mixture was stirred for 2 hours at 100° C. After cooling, and removal of the volatiles ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2ncccc2c1.c1ccc2ncncc2c1.C1CC[NH]CC1
HCl
CN(C)C=O
100
2
COc1cc2c(Cl)ncnc2cc1OCC1CCN(CCS(C)(=O)=O)CC1.Oc1ccc2cccnc2c1>CN(C)C=O>COc1cc2c(Oc3ccc4cccnc4c3)ncnc2cc1OCC1CCN(CCS(C)(=O)=O)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4c6833833a84432693784735392fb8a4
CC(C)(C)C(=O)OCCl.COc1cc2c(=O)[nH]cnc2cc1OCc1ccccc1>>COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCc1ccccc1
C(C(C)(C)C)(=O)OCCl.[H-].[Na+].C(C1=CC=CC=C1)OC1=C(C=C2C(NC=NC2=C1)=O)OC.Cl>>C(C1=CC=CC=C1)OC1=C(C=C2C(N(C=NC2=C1)COC(C(C)(C)C)=O)=O)OC
Cl[CH2:9][O:10][C:11](=[O:12])[C:13]([CH3:14])([CH3:15])[CH3:16].[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6](=[O:7])[nH:8][cH:17][n:18][c:19]2[cH:20][c:21]1[O:22][CH2:23][c:24]1[cH:25][cH:26][cH:27][cH:28][cH:29]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6](=[O:7])[n:8]([CH2:9][O:10][C:11](=[O:12])[C:13]([CH3:14])([CH3:15])[CH3:16])[...
CC(C)(C)C(=O)OCCl.COc1cc2c(=O)[nH]cnc2cc1OCc1ccccc1
COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCc1ccccc1
null
null
CN(C)C=O.C(C)(=O)OCC
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
3356b731e3fd312a1caad9e7f3379edf1f464b4ff06052540679496363168d0d
6007d70cc3173f3039a472489995dad2781e8d749be1f1aa209b0bf2f190a4b4
O=c1[nH]cnc2cc(OCc3ccccc3)ccc12
Cl-[CH2;D2;+0:1]-[#8:2]-[C:3](-[C:4])=[O;D1;H0:5].[O;D1;H0:6]=[c:7]1:[c:8]:[c:9]:[#7;a:10]:[c:11]:[nH;D2;+0:12]:1>>[C:4]-[C:3](=[O;D1;H0:5])-[#8:2]-[CH2;D2;+0:1]-[n;H0;D3;+0:12]1:[c:11]:[#7;a:10]:[c:9]:[c:8]:[c:7]:1=[O;D1;H0:6]
84.1
[{"value": 84.0, "product": "C(C1=CC=CC=C1)OC1=C(C=C2C(N(C=NC2=C1)COC(C(C)(C)C)=O)=O)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 84.1, "product": "C(C1=CC=CC=C1)OC1=C(C=C2C(N(C=NC2=C1)COC(C(C)(C)C)=O)=O)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1.5
HOUR
Sodium hydride (1.44 g of a 60% suspension in mineral oil, 36 mmol) was added in portions over 20 minutes to a solution of 7-benzyloxy-6-methoxy-3,4-dihydroquinazolin-4-one (8.46 g, 30 mmol), (prepared as described for the starting material in Example 1), in DMF (70 ml) and the mixture was stirred for 1.5 hours. Chloro...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester
Ester
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2ncncc2c1.c1ccccc1
HCl
CN(C)C=O.C(C)(=O)OCC
null
1.5
CC(C)(C)C(=O)OCCl.COc1cc2c(=O)[nH]cnc2cc1OCc1ccccc1>CN(C)C=O.C(C)(=O)OCC>COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCc1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-105dd76d5f2344198beb01fbd2071e55
COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCc1ccccc1>>COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1O
C(C1=CC=CC=C1)OC1=C(C=C2C(N(C=NC2=C1)COC(C(C)(C)C)=O)=O)OC>>OC1=C(C=C2C(N(C=NC2=C1)COC(C(C)(C)C)=O)=O)OC
c1ccc(C[O:22][c:21]2[c:3]([O:2][CH3:1])[cH:4][c:5]3[c:6](=[O:7])[n:8]([CH2:9][O:10][C:11](=[O:12])[C:13]([CH3:14])([CH3:15])[CH3:16])[cH:17][n:18][c:19]3[cH:20]2)cc1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6](=[O:7])[n:8]([CH2:9][O:10][C:11](=[O:12])[C:13]([CH3:14])([CH3:15])[CH3:16])[cH:17][n:18][c:19]2[cH:20][c:21]1[OH:22]
COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCc1ccccc1
COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1O
null
[Pd]
CO.C(C)(=O)O.CN(C)C=O.C(C)(=O)OCC
Deprotection
Hydroxyl benzyl deprotection
36869d1fe85185a14d9eb30bf05178c600a9b6eca277ffaf3803578c30e0bf5d
26a36596df80ec137b0e8087297418351c93c32819177f680675220622f215d4
O=c1[nH]cnc2ccccc12
[#7;a:1]:[c:2]:[c:3]:[c:4](-[O;H0;D2;+0:5]-C-c1:c:c:c:c:c:1):[c:6]>>[#7;a:1]:[c:2]:[c:3]:[c:4](-[OH;D1;+0:5]):[c:6]
80.4
[{"value": 80.0, "product": "OC1=C(C=C2C(N(C=NC2=C1)COC(C(C)(C)C)=O)=O)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 80.4, "product": "OC1=C(C=C2C(N(C=NC2=C1)COC(C(C)(C)C)=O)=O)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
40
MINUTE
A mixture of 7-benzyloxy-6-methoxy-3-((pivaloyloxy)methyl)-3,4-dihydroquinazolin-4-one (7 g, 17.7 mmol) and 10% palladium-on-charcoal catalyst (700 mg) in ethyl acetate (250 ml), DMF (50 ml), methanol (50 ml) and acetic acid (0.7 ml) was stirred under hydrogen at atmospheric pressure for 40 minutes. The catalyst was re...
10.6084/m9.figshare.5104873.v1
null
Ether
Aromatic alcohol
c1ccccc1
null
c1ccc2ncncc2c1
Other
[Pd].CO.C(C)(=O)O.CN(C)C=O.C(C)(=O)OCC
null
0.666667
COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCc1ccccc1>[Pd].CO.C(C)(=O)O.CN(C)C=O.C(C)(=O)OCC>COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-8ccda9cb1d66403782b1f8739af8d082
COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1O.Cc1ccc(S(=O)(=O)OCC2CCN(C(=O)OC(C)(C)C)CC2)cc1>>COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCC1CCN(C(=O)OC(C)(C)C)CC1
OC1=C(C=C2C(N(C=NC2=C1)COC(C(C)(C)C)=O)=O)OC.CC1=CC=C(C=C1)S(=O)(=O)OCC1CCN(CC1)C(=O)OC(C)(C)C.Cl>>COC=1C=C2C(N(C=NC2=CC1OCC1CCN(CC1)C(=O)OC(C)(C)C)COC(C(C)(C)C)=O)=O
[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6](=[O:7])[n:8]([CH2:9][O:10][C:11](=[O:12])[C:13]([CH3:14])([CH3:15])[CH3:16])[cH:17][n:18][c:19]2[cH:20][c:21]1[OH:22].Cc1ccc(S(=O)(=O)O[CH2:23][CH:24]2[CH2:25][CH2:26][N:27]([C:28](=[O:29])[O:30][C:31]([CH3:32])([CH3:33])[CH3:34])[CH2:35][CH2:36]2)cc1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[...
COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1O.Cc1ccc(S(=O)(=O)OCC2CCN(C(=O)OC(C)(C)C)CC2)cc1
COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCC1CCN(C(=O)OC(C)(C)C)CC1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
OtherReaction
b5213736859cf91483a02f350869986d9b7674724716adef8a5d7a4bbdb79574
3d107e624e135e10014c7bf413dd0be27e1e4488f039e545b94cb1680b764158
O=c1[nH]cnc2cc(OCC3CCNCC3)ccc12
C-c1:c:c:c(-S(=O)(=O)-O-[CH2;D2;+0:1]-[C:2](-[C:3])-[C:4]):c:c:1.[#7;a:5]:[c:6]:[c:7]:[c:8](-[OH;D1;+0:9]):[c:10]>>[#7;a:5]:[c:6]:[c:7]:[c:8](-[O;H0;D2;+0:9]-[CH2;D2;+0:1]-[C:2](-[C:3])-[C:4]):[c:10]
78.5
[{"value": 78.5, "product": "COC=1C=C2C(N(C=NC2=CC1OCC1CCN(CC1)C(=O)OC(C)(C)C)COC(C(C)(C)C)=O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 78.4, "product": "COC=1C=C2C(N(C=NC2=CC1OCC1CCN(CC1)C(=O)OC(C)(C)C)COC(C(C)(C)C)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
A suspension of 7-hydroxy-6-methoxy-3-((pivaloyloxy)methyl)-3,4-dihydroquinazolin-4-one (6.12 g, 20 mmol) potassium carbonate (5.52 g, 40 mmol) in DMF (60 ml) was stirred at ambient temperature for 30 minutes. 4-(4-Methylphenylsulphonyloxymethyl)-1-tert-butyloxycarbonylpiperidine (8.86 g, 24 mmol), (prepared as describ...
10.6084/m9.figshare.5104873.v1
null
Tosylate.Aromatic alcohol
Ether
c1ccccc1
null
c1ccc2ncncc2c1.C1CC[NH]CC1
TsOH.HO-
CN(C)C=O
null
0.5
COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1O.Cc1ccc(S(=O)(=O)OCC2CCN(C(=O)OC(C)(C)C)CC2)cc1>CN(C)C=O>COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCC1CCN(C(=O)OC(C)(C)C)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-95eea2a3d9644b2091926b32c1b9b868
COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCC1CCN(C(=O)OC(C)(C)C)CC1>>COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCC1CCNCC1
COC=1C=C2C(N(C=NC2=CC1OCC1CCN(CC1)C(=O)OC(C)(C)C)COC(C(C)(C)C)=O)=O.Cl.CCOCC>>Cl.COC=1C=C2C(N(C=NC2=CC1OCC1CCNCC1)COC(C(C)(C)C)=O)=O
CC(C)(C)OC(=O)[N:27]1[CH2:26][CH2:25][CH:24]([CH2:23][O:22][c:21]2[c:3]([O:2][CH3:1])[cH:4][c:5]3[c:6](=[O:7])[n:8]([CH2:9][O:10][C:11](=[O:12])[C:13]([CH3:14])([CH3:15])[CH3:16])[cH:17][n:18][c:19]3[cH:20]2)[CH2:29][CH2:28]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6](=[O:7])[n:8]([CH2:9][O:10][C:11](=[O:12])[C:13]([CH3:14])...
COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCC1CCN(C(=O)OC(C)(C)C)CC1
COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCC1CCNCC1
null
null
C(C)(C)O.C(Cl)Cl
Reduction
Boc amine deprotection
bf3cd5dc3e17e694d8665c89f5d7e08e8763b18436a633eb66e9bf530b8b0316
a94b29c7264c852156fc1cdd4a0951a4fc26c06d0edc9e50c743825dbf79e3fd
O=c1[nH]cnc2cc(OCC3CCNCC3)ccc12
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1](-[C:2]-[C:3])-[C:4]-[C:5]>>[C:3]-[C:2]-[NH;D2;+0:1]-[C:4]-[C:5]
100
[{"value": 100.0, "product": "Cl.COC=1C=C2C(N(C=NC2=CC1OCC1CCNCC1)COC(C(C)(C)C)=O)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
A solution of 6-methoxy-3-((pivaloyloxy)methyl)-7-((1-tert-butyloxycarbonylpiperidin-4-yl)methoxy)-3,4-dihydroquinazolin-4-one (7.9 g, 16 mmol) in methylene chloride (80 ml) containing 5.5M hydrogen chloride in isopropanol (80 ml) was stirred for 1 hour at ambient temperature. Ether was added and the solid was collecte...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Secondary amine
C1CC[NH]CC1
C1CCNCC1
c1ccc2ncncc2c1.C1CCNCC1
HO-
C(C)(C)O.C(Cl)Cl
null
1
COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCC1CCN(C(=O)OC(C)(C)C)CC1>C(C)(C)O.C(Cl)Cl>COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCC1CCNCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e3beac8f71b2485eb4b26f8397efafc2
C=CS(C)(=O)=O.COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCC1CCNCC1>>COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCC1CCN(CCS(C)(=O)=O)CC1
Cl.COC=1C=C2C(N(C=NC2=CC1OCC1CCNCC1)COC(C(C)(C)C)=O)=O.C(C)N(CC)CC.C([O-])([O-])=O.[K+].[K+].C(=C)S(=O)(=O)C>>COC=1C=C2C(N(C=NC2=CC1OCC1CCN(CC1)CCS(=O)(=O)C)COC(C(C)(C)C)=O)=O
[CH2:28]=[CH:29][S:30]([CH3:31])(=[O:32])=[O:33].[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6](=[O:7])[n:8]([CH2:9][O:10][C:11](=[O:12])[C:13]([CH3:14])([CH3:15])[CH3:16])[cH:17][n:18][c:19]2[cH:20][c:21]1[O:22][CH2:23][CH:24]1[CH2:25][CH2:26][NH:27][CH2:34][CH2:35]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6](=[O:7])[n:8]([CH2:9][O:10...
C=CS(C)(=O)=O.COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCC1CCNCC1
COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCC1CCN(CCS(C)(=O)=O)CC1
null
null
C(Cl)Cl.CO
Heteroatom Alkylation and Arylation
aza-Michael addition secondary
d3e8cc768c824777b70742851768dcb27bf5f461c310912ac3f5a7abd08f6975
828fcbb87adfef9f22c9a1e52b43c3df76cb2e49bfe62b57e8b79965772a2bed
O=c1[nH]cnc2cc(OCC3CCNCC3)ccc12
[C;D1;H3:1]-[#16:2](=[O;D1;H0:3])(=[O;D1;H0:4])-[CH;D2;+0:5]=[CH2;D1;+0:6].[C:7]-[C:8]-[NH;D2;+0:9]-[C:10]-[C:11]>>[C:7]-[C:8]-[N;H0;D3;+0:9](-[CH2;D2;+0:6]-[CH2;D2;+0:5]-[#16:2](-[C;D1;H3:1])(=[O;D1;H0:3])=[O;D1;H0:4])-[C:10]-[C:11]
54
[{"value": 54.0, "product": "COC=1C=C2C(N(C=NC2=CC1OCC1CCN(CC1)CCS(=O)(=O)C)COC(C(C)(C)C)=O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 54.0, "product": "COC=1C=C2C(N(C=NC2=CC1OCC1CCN(CC1)CCS(=O)(=O)C)COC(C(C)(C)C)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
To a solution of 6-methoxy-7-((piperidin-4-yl)methoxy)-3-((pivaloyloxy)methyl)-3,4-dihydroquinazolin-4-one hydrochloride (0.88 g, 2 mmol) and triethylamine (0.3 ml, 2.1 mmol) in methanol (10 ml) and methylene chloride (10 ml) was added potassium carbonate (280 mg, 2 mmol) and methyl vinyl sulfone (0.4 ml, 2.1 mmol). Af...
10.6084/m9.figshare.5104873.v1
null
Secondary amine.Vinyl
Tertiary amine
C1CCNCC1
C1CC[NH]CC1
c1ccc2ncncc2c1.C1CC[NH]CC1
null
C(Cl)Cl.CO
null
2
C=CS(C)(=O)=O.COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCC1CCNCC1>C(Cl)Cl.CO>COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCC1CCN(CCS(C)(=O)=O)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c855e264da9645dab49f60f7290300d3
COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCC1CCN(CCS(C)(=O)=O)CC1>>COc1cc2c(=O)[nH]cnc2cc1OCC1CCN(CCS(C)(=O)=O)CC1
Cl.[OH-].[Na+].COC=1C=C2C(N(C=NC2=CC1OCC1CCN(CC1)CCS(=O)(=O)C)COC(C(C)(C)C)=O)=O.CC1=CC=C(C=C1)COC(=O)NNC(=O)C2=NC=CN=C2>>COC=1C=C2C(NC=NC2=CC1OCC1CCN(CC1)CCS(=O)(=O)C)=O
CC(C)(C)C(=O)OC[n:8]1[c:6](=[O:7])[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:13]([O:14][CH2:15][CH:16]3[CH2:17][CH2:18][N:19]([CH2:20][CH2:21][S:22]([CH3:23])(=[O:24])=[O:25])[CH2:26][CH2:27]3)[cH:12][c:11]2[n:10][cH:9]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6](=[O:7])[nH:8][cH:9][n:10][c:11]2[cH:12][c:13]1[O:14][CH2:15][CH:16]1[CH...
COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCC1CCN(CCS(C)(=O)=O)CC1
COc1cc2c(=O)[nH]cnc2cc1OCC1CCN(CCS(C)(=O)=O)CC1
null
null
CO
Reduction
OtherReaction
9f6991089c15fc054898797f1d3a42b158e517f125611bc103acfc00878b3b20
b8e5da8ea19c403a2e974791a9cf591400749acb6b71151717aaece4f3b22bef
O=c1[nH]cnc2cc(OCC3CCNCC3)ccc12
C-C(-C)(-C)-C(=O)-O-C-[n;H0;D3;+0:1]1:[c:2]:[#7;a:3]:[c:4]:[c:5]:[c:6]:1=[O;D1;H0:7]>>[O;D1;H0:7]=[c:6]1:[c:5]:[c:4]:[#7;a:3]:[c:2]:[nH;D2;+0:1]:1
79
[{"value": 79.0, "product": "COC=1C=C2C(NC=NC2=CC1OCC1CCN(CC1)CCS(=O)(=O)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 77.3, "product": "COC=1C=C2C(NC=NC2=CC1OCC1CCN(CC1)CCS(=O)(=O)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
To a suspension of 6-methoxy-7-((1-(2-methylsulphonylethyl)piperidin-4-yl)methoxy)-3-((pivaloyloxy)methyl)-3,4-dihydroquinazolin-4-one (90 mg, 0.18 mmol) in methanol (3 ml) was added 2M aqueous sodium hydroxide (180 μl, 0.35 mmol). After stirring for 2 hours at ambient temperature, the mixture was adjusted to pH10 with...
10.6084/m9.figshare.5104873.v1
null
Ester
null
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2ncncc2c1.C1CC[NH]CC1
HO-
CO
null
2
COc1cc2c(=O)n(COC(=O)C(C)(C)C)cnc2cc1OCC1CCN(CCS(C)(=O)=O)CC1>CO>COc1cc2c(=O)[nH]cnc2cc1OCC1CCN(CCS(C)(=O)=O)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f47b2f24d0d24ae8bfeb5a625660c16e
COc1cc2c(Cl)ncnc2cc1OCC1CCN(C)CC1.Cc1ccnc2cc(O)ccc12>>COc1cc2c(Oc3ccc4c(C)ccnc4c3)ncnc2cc1OCC1CCN(C)CC1
ClC1=NC=NC2=CC(=C(C=C12)OC)OCC1CCN(CC1)C.CC1=CC=NC2=CC(=CC=C12)O>>COC=1C=C2C(=NC=NC2=CC1OCC1CCN(CC1)C)OC1=CC=C2C(=CC=NC2=C1)C
Cl[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:24]([O:25][CH2:26][CH:27]3[CH2:28][CH2:29][N:30]([CH3:31])[CH2:32][CH2:33]3)[cH:23][c:22]2[n:21][cH:20][n:19]1.[OH:7][c:8]1[cH:9][cH:10][c:11]2[c:12]([CH3:13])[cH:14][cH:15][n:16][c:17]2[cH:18]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([O:7][c:8]3[cH:9][cH:10][c:11]4[c:12]([CH3:13]...
COc1cc2c(Cl)ncnc2cc1OCC1CCN(C)CC1.Cc1ccnc2cc(O)ccc12
COc1cc2c(Oc3ccc4c(C)ccnc4c3)ncnc2cc1OCC1CCN(C)CC1
null
null
null
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
2d25b59c80a437134e7830160726da4e12ee4089c37759035843c1cccd8cd262
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1cnc2cc(Oc3ncnc4cc(OCC5CCNCC5)ccc34)ccc2c1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[#7;a:9]:[c:10]:[c:11]:[c:12](-[OH;D1;+0:13]):[c:14]>>[#7;a:9]:[c:10]:[c:11]:[c:12](-[O;H0;D2;+0:13]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8]):[c:14]
90
[{"value": 90.0, "product": "COC=1C=C2C(=NC=NC2=CC1OCC1CCN(CC1)C)OC1=CC=C2C(=CC=NC2=C1)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 90.0, "product": "COC=1C=C2C(=NC=NC2=CC1OCC1CCN(CC1)C)OC1=CC=C2C(=CC=NC2=C1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Using a procedure analogous to that described for Example 10, 4-chloro-6-methoxy-7-((1-methylpiperidin-4-yl)methoxy)quinazoline (130 mg, 0.4 mmol), (prepared as described for the starting material in Example 10), was reacted with 4-methyl-7-hydroxyquinoline (80 mg, 0.5 mol), (Chem. Ber. 1967, 100, 2077), to give 6-meth...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2ncccc2c1.c1ccc2ncncc2c1.C1CC[NH]CC1
HCl
null
null
null
COc1cc2c(Cl)ncnc2cc1OCC1CCN(C)CC1.Cc1ccnc2cc(O)ccc12>>COc1cc2c(Oc3ccc4c(C)ccnc4c3)ncnc2cc1OCC1CCN(C)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-00698d5f0e3b424b91f30a1c746a1b8d
COc1cc2c(Cl)ncnc2cc1OCC1CCN(CCS(C)(=O)=O)CC1.Cc1cc2cc(O)ccc2[nH]1>>COc1cc2c(Oc3ccc4[nH]c(C)cc4c3)ncnc2cc1OCC1CCN(CCS(C)(=O)=O)CC1
ClC1=NC=NC2=CC(=C(C=C12)OC)OCC1CCN(CC1)CCS(=O)(=O)C.OC=1C=C2C=C(NC2=CC1)C.C([O-])([O-])=O.[K+].[K+]>>COC=1C=C2C(=NC=NC2=CC1OCC1CCN(CC1)CCS(=O)(=O)C)OC=1C=C2C=C(NC2=CC1)C
Cl[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:23]([O:24][CH2:25][CH:26]3[CH2:27][CH2:28][N:29]([CH2:30][CH2:31][S:32]([CH3:33])(=[O:34])=[O:35])[CH2:36][CH2:37]3)[cH:22][c:21]2[n:20][cH:19][n:18]1.[OH:7][c:8]1[cH:9][cH:10][c:11]2[nH:12][c:13]([CH3:14])[cH:15][c:16]2[cH:17]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([O:7][c:8]3[...
COc1cc2c(Cl)ncnc2cc1OCC1CCN(CCS(C)(=O)=O)CC1.Cc1cc2cc(O)ccc2[nH]1
COc1cc2c(Oc3ccc4[nH]c(C)cc4c3)ncnc2cc1OCC1CCN(CCS(C)(=O)=O)CC1
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
2d25b59c80a437134e7830160726da4e12ee4089c37759035843c1cccd8cd262
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1nc(Oc2ccc3[nH]ccc3c2)c2ccc(OCC3CCNCC3)cc2n1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[OH;D1;+0:9]-[c:10](:[c:11]):[c:12]>>[c:11]:[c:10](-[O;H0;D2;+0:9]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8]):[c:12]
41
[{"value": 41.0, "product": "COC=1C=C2C(=NC=NC2=CC1OCC1CCN(CC1)CCS(=O)(=O)C)OC=1C=C2C=C(NC2=CC1)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 40.8, "product": "COC=1C=C2C(=NC=NC2=CC1OCC1CCN(CC1)CCS(=O)(=O)C)OC=1C=C2C=C(NC2=CC1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
2
HOUR
A solution of 4-chloro-6-methoxy-7-((1-(2-methylsulphonylethyl)piperidin-4-yl)methoxy)quinazoline (115 mg, 0.28 mmol), (prepared as described for the starting material in Example 12), 5-hydroxy-2-methylindole (50 mg, 0.33 mmol) and potassium carbonate (60 mg, 0.42 mmol) in DMF (1.5 ml) was stirred at 100° C. for 2 hour...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2[nH]ccc2c1.c1ccc2ncncc2c1.C1CC[NH]CC1
HCl
CN(C)C=O
100
2
COc1cc2c(Cl)ncnc2cc1OCC1CCN(CCS(C)(=O)=O)CC1.Cc1cc2cc(O)ccc2[nH]1>CN(C)C=O>COc1cc2c(Oc3ccc4[nH]c(C)cc4c3)ncnc2cc1OCC1CCN(CCS(C)(=O)=O)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-01a9ce6cc8a944af8a778180893ea3e8
COc1cc2c(Cl)ncnc2cc1OCCCN1CCCC1.Cc1ccnc2cc(O)ccc12>>COc1cc2c(Oc3ccc4c(C)ccnc4c3)ncnc2cc1OCCCN1CCCC1
ClC1=NC=NC2=CC(=C(C=C12)OC)OCCCN1CCCC1.OC1=CC=C2C(=CC=NC2=C1)C>>COC=1C=C2C(=NC=NC2=CC1OCCCN1CCCC1)OC1=CC=C2C(=CC=NC2=C1)C
Cl[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:24]([O:25][CH2:26][CH2:27][CH2:28][N:29]3[CH2:30][CH2:31][CH2:32][CH2:33]3)[cH:23][c:22]2[n:21][cH:20][n:19]1.[OH:7][c:8]1[cH:9][cH:10][c:11]2[c:12]([CH3:13])[cH:14][cH:15][n:16][c:17]2[cH:18]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([O:7][c:8]3[cH:9][cH:10][c:11]4[c:12]([CH3:13])...
COc1cc2c(Cl)ncnc2cc1OCCCN1CCCC1.Cc1ccnc2cc(O)ccc12
COc1cc2c(Oc3ccc4c(C)ccnc4c3)ncnc2cc1OCCCN1CCCC1
null
null
null
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
2d25b59c80a437134e7830160726da4e12ee4089c37759035843c1cccd8cd262
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1cnc2cc(Oc3ncnc4cc(OCCCN5CCCC5)ccc34)ccc2c1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[#7;a:9]:[c:10]:[c:11]:[c:12](-[OH;D1;+0:13]):[c:14]>>[#7;a:9]:[c:10]:[c:11]:[c:12](-[O;H0;D2;+0:13]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8]):[c:14]
87.2
[{"value": 87.0, "product": "COC=1C=C2C(=NC=NC2=CC1OCCCN1CCCC1)OC1=CC=C2C(=CC=NC2=C1)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 87.2, "product": "COC=1C=C2C(=NC=NC2=CC1OCCCN1CCCC1)OC1=CC=C2C(=CC=NC2=C1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Using a procedure analogous to that described for Example 9, 4-chloro-6-methoxy-7-(3-(pyrrolidin-1-yl)propoxy)quinazoline (0.13 g, 0.4 mmol), (prepared as described for the starting material in Example 9), was reacted with 7-hydroxy-4-methylquinoline (80 mg, 0.5 mol), (Chem. Berich. 1967, 100, 2077), to give 6-methoxy-...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2ncccc2c1.c1ccc2ncncc2c1.C1CC[NH]C1
HCl
null
null
null
COc1cc2c(Cl)ncnc2cc1OCCCN1CCCC1.Cc1ccnc2cc(O)ccc12>>COc1cc2c(Oc3ccc4c(C)ccnc4c3)ncnc2cc1OCCCN1CCCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-7cc1b1fbb9924b418ed5c2868d74e86d
CC1=CC(C)(C)Nc2ccc(O)cc21.COc1cc2c(Cl)ncnc2cc1OCCCN1CCCC1>>COc1cc2c(Oc3ccc4c(c3)C(C)=CC(C)(C)N4)ncnc2cc1OCCCN1CCCC1
ClC1=NC=NC2=CC(=C(C=C12)OC)OCCCN1CCCC1.CC1(NC2=CC=C(C=C2C(=C1)C)O)C>>COC=1C=C2C(=NC=NC2=CC1OCCCN1CCCC1)OC=1C=C2C(=CC(NC2=CC1)(C)C)C
[OH:7][c:8]1[cH:9][cH:10][c:11]2[c:12]([cH:13]1)[C:14]([CH3:15])=[CH:16][C:17]([CH3:18])([CH3:19])[NH:20]2.Cl[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:26]([O:27][CH2:28][CH2:29][CH2:30][N:31]3[CH2:32][CH2:33][CH2:34][CH2:35]3)[cH:25][c:24]2[n:23][cH:22][n:21]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([O:7][c:8]3[cH:9][cH:10]...
CC1=CC(C)(C)Nc2ccc(O)cc21.COc1cc2c(Cl)ncnc2cc1OCCCN1CCCC1
COc1cc2c(Oc3ccc4c(c3)C(C)=CC(C)(C)N4)ncnc2cc1OCCCN1CCCC1
null
null
null
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
2d25b59c80a437134e7830160726da4e12ee4089c37759035843c1cccd8cd262
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
C1=Cc2cc(Oc3ncnc4cc(OCCCN5CCCC5)ccc34)ccc2NC1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[OH;D1;+0:9]-[c:10](:[c:11]):[c:12]>>[c:11]:[c:10](-[O;H0;D2;+0:9]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8]):[c:12]
47.4
[{"value": 47.0, "product": "COC=1C=C2C(=NC=NC2=CC1OCCCN1CCCC1)OC=1C=C2C(=CC(NC2=CC1)(C)C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 47.4, "product": "COC=1C=C2C(=NC=NC2=CC1OCCCN1CCCC1)OC=1C=C2C(=CC(NC2=CC1)(C)C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Using a procedure analogous to that described for Example 9, 4-chloro-6-methoxy-7-(3-(pyrrolidin-1-yl)propoxy)quinazoline (0.13 g, 0.4 mmol), (prepared as described for the starting material in Example 9), was reacted with 2,2,4-trimethyl-1,2-dihydroquinolin-6-ol (95 mg, 0.5 mmol), (IZV. ACAD. NAVK. SSSR. Ser. Khim. 19...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccc2ncncc2c1
c1ccc2ncncc2c1
C1=Cc2ccccc2NC1.c1ccc2ncncc2c1.C1CC[NH]C1
HCl
null
null
null
CC1=CC(C)(C)Nc2ccc(O)cc21.COc1cc2c(Cl)ncnc2cc1OCCCN1CCCC1>>COc1cc2c(Oc3ccc4c(c3)C(C)=CC(C)(C)N4)ncnc2cc1OCCCN1CCCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-04c6877b345344b1a4dc437ccebfe1b6
CC1=CC(C)(C)Nc2ccc(O)cc21.COc1cc2c(Cl)ncnc2cc1OCC1CCN(C)CC1>>COc1cc2c(Oc3ccc4c(c3)C(C)=CC(C)(C)N4)ncnc2cc1OCC1CCN(C)CC1
ClC1=NC=NC2=CC(=C(C=C12)OC)OCC1CCN(CC1)C.CC1(NC2=CC=C(C=C2C(=C1)C)O)C>>COC=1C=C2C(=NC=NC2=CC1OCC1CCN(CC1)C)OC=1C=C2C(=CC(NC2=CC1)(C)C)C
[OH:7][c:8]1[cH:9][cH:10][c:11]2[c:12]([cH:13]1)[C:14]([CH3:15])=[CH:16][C:17]([CH3:18])([CH3:19])[NH:20]2.Cl[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:26]([O:27][CH2:28][CH:29]3[CH2:30][CH2:31][N:32]([CH3:33])[CH2:34][CH2:35]3)[cH:25][c:24]2[n:23][cH:22][n:21]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([O:7][c:8]3[cH:9][cH:10...
CC1=CC(C)(C)Nc2ccc(O)cc21.COc1cc2c(Cl)ncnc2cc1OCC1CCN(C)CC1
COc1cc2c(Oc3ccc4c(c3)C(C)=CC(C)(C)N4)ncnc2cc1OCC1CCN(C)CC1
null
null
null
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
2d25b59c80a437134e7830160726da4e12ee4089c37759035843c1cccd8cd262
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
C1=Cc2cc(Oc3ncnc4cc(OCC5CCNCC5)ccc34)ccc2NC1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[OH;D1;+0:9]-[c:10](:[c:11]):[c:12]>>[c:11]:[c:10](-[O;H0;D2;+0:9]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8]):[c:12]
74
[{"value": 74.0, "product": "COC=1C=C2C(=NC=NC2=CC1OCC1CCN(CC1)C)OC=1C=C2C(=CC(NC2=CC1)(C)C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 73.7, "product": "COC=1C=C2C(=NC=NC2=CC1OCC1CCN(CC1)C)OC=1C=C2C(=CC(NC2=CC1)(C)C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Using a procedure analogous to that described for Example 9, 4-chloro-6-methoxy-7-((1-methylpiperidin-4-yl)methoxy)quinazoline (0.13 g, 0.4 mmol), (prepared as described for the starting material in Example 10), was reacted with 2,2,4-trimethyl-1,2-dihydroquinolin-6-ol (95 mg, 0.5 mmol), (IZV. ACAD. NAVK. SSSR. Ser. Kh...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccc2ncncc2c1
c1ccc2ncncc2c1
C1=Cc2ccccc2NC1.c1ccc2ncncc2c1.C1CC[NH]CC1
HCl
null
null
null
CC1=CC(C)(C)Nc2ccc(O)cc21.COc1cc2c(Cl)ncnc2cc1OCC1CCN(C)CC1>>COc1cc2c(Oc3ccc4c(c3)C(C)=CC(C)(C)N4)ncnc2cc1OCC1CCN(C)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-03499002c4e144409125c00cc7f18366
COc1cc2c(Cl)ncnc2cc1OCC1CCN(C)CC1.Cc1cc(C)c2ccc(O)cc2n1>>COc1cc2c(Oc3ccc4c(C)cc(C)nc4c3)ncnc2cc1OCC1CCN(C)CC1
ClC1=NC=NC2=CC(=C(C=C12)OC)OCC1CCN(CC1)C.CC1=NC2=CC(=CC=C2C(=C1)C)O>>CC1=NC2=CC(=CC=C2C(=C1)C)OC1=NC=NC2=CC(=C(C=C12)OC)OCC1CCN(CC1)C
Cl[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:25]([O:26][CH2:27][CH:28]3[CH2:29][CH2:30][N:31]([CH3:32])[CH2:33][CH2:34]3)[cH:24][c:23]2[n:22][cH:21][n:20]1.[OH:7][c:8]1[cH:9][cH:10][c:11]2[c:12]([CH3:13])[cH:14][c:15]([CH3:16])[n:17][c:18]2[cH:19]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([O:7][c:8]3[cH:9][cH:10][c:11]4[c:12]...
COc1cc2c(Cl)ncnc2cc1OCC1CCN(C)CC1.Cc1cc(C)c2ccc(O)cc2n1
COc1cc2c(Oc3ccc4c(C)cc(C)nc4c3)ncnc2cc1OCC1CCN(C)CC1
null
null
null
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
2d25b59c80a437134e7830160726da4e12ee4089c37759035843c1cccd8cd262
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1cnc2cc(Oc3ncnc4cc(OCC5CCNCC5)ccc34)ccc2c1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[#7;a:9]:[c:10]:[c:11]:[c:12](-[OH;D1;+0:13]):[c:14]>>[#7;a:9]:[c:10]:[c:11]:[c:12](-[O;H0;D2;+0:13]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8]):[c:14]
33.3
[{"value": 33.0, "product": "CC1=NC2=CC(=CC=C2C(=C1)C)OC1=NC=NC2=CC(=C(C=C12)OC)OCC1CCN(CC1)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 33.3, "product": "CC1=NC2=CC(=CC=C2C(=C1)C)OC1=NC=NC2=CC(=C(C=C12)OC)OCC1CCN(CC1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Using a procedure analogous to that described for Example 9, 4-chloro-6-methoxy-7-((1-methylpiperidin-4-yl)methoxy)quinazoline (0.13 g, 0.4 mmol), (prepared as described for the starting material in Example 10), was reacted with 2,4-dimethyl-7-hydroxyquinoline (87 mg, 0.5 mmol), (Chem. Berichte, 1903, 36, 4016), to giv...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2ncccc2c1.c1ccc2ncncc2c1.C1CC[NH]CC1
HCl
null
null
null
COc1cc2c(Cl)ncnc2cc1OCC1CCN(C)CC1.Cc1cc(C)c2ccc(O)cc2n1>>COc1cc2c(Oc3ccc4c(C)cc(C)nc4c3)ncnc2cc1OCC1CCN(C)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5a514b9975c547d895e0fc229b7da49d
COc1cc2c(Cl)ncnc2cc1OCC1CCN(C)CC1.O=C1COc2ccc(O)cc2N1>>COc1cc2c(Oc3ccc4c(c3)NC(=O)CO4)ncnc2cc1OCC1CCN(C)CC1
ClC1=NC=NC2=CC(=C(C=C12)OC)OCC1CCN(CC1)C.OC=1C=CC2=C(NC(CO2)=O)C1>>COC=1C=C2C(=NC=NC2=CC1OCC1CCN(CC1)C)OC=1C=CC2=C(NC(CO2)=O)C1
Cl[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:24]([O:25][CH2:26][CH:27]3[CH2:28][CH2:29][N:30]([CH3:31])[CH2:32][CH2:33]3)[cH:23][c:22]2[n:21][cH:20][n:19]1.[OH:7][c:8]1[cH:9][cH:10][c:11]2[c:12]([cH:13]1)[NH:14][C:15](=[O:16])[CH2:17][O:18]2>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([O:7][c:8]3[cH:9][cH:10][c:11]4[c:12]([cH:13...
COc1cc2c(Cl)ncnc2cc1OCC1CCN(C)CC1.O=C1COc2ccc(O)cc2N1
COc1cc2c(Oc3ccc4c(c3)NC(=O)CO4)ncnc2cc1OCC1CCN(C)CC1
null
null
null
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
2d25b59c80a437134e7830160726da4e12ee4089c37759035843c1cccd8cd262
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
O=C1COc2ccc(Oc3ncnc4cc(OCC5CCNCC5)ccc34)cc2N1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[OH;D1;+0:9]-[c:10](:[c:11]):[c:12]>>[c:11]:[c:10](-[O;H0;D2;+0:9]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8]):[c:12]
88
[{"value": 88.0, "product": "COC=1C=C2C(=NC=NC2=CC1OCC1CCN(CC1)C)OC=1C=CC2=C(NC(CO2)=O)C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 87.7, "product": "COC=1C=C2C(=NC=NC2=CC1OCC1CCN(CC1)C)OC=1C=CC2=C(NC(CO2)=O)C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Using a procedure analogous to that described for Example 9, 4-chloro-6-methoxy-7-((1-methylpiperidin-4-yl)methoxy)quinazoline (0.13 g, 0.4 mmol), (prepared as described for the starting material in Example 10), was reacted with 6-hydroxy-2H-4H-1,4-benzoxazin-3-one (83 mg, 0.5 mmol), (J. Chem. Soc. C, 1971, 2696), to g...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2c(c1)NCCO2.c1ccc2ncncc2c1.C1CC[NH]CC1
HCl
null
null
null
COc1cc2c(Cl)ncnc2cc1OCC1CCN(C)CC1.O=C1COc2ccc(O)cc2N1>>COc1cc2c(Oc3ccc4c(c3)NC(=O)CO4)ncnc2cc1OCC1CCN(C)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-45e1fb03180e465799ca19177569b4db
COc1cc2c(Cl)ncnc2cc1OCCCN1CCCC1.O=C1COc2ccc(O)cc2N1>>COc1cc2c(Oc3ccc4c(c3)NC(=O)CO4)ncnc2cc1OCCCN1CCCC1
ClC1=NC=NC2=CC(=C(C=C12)OC)OCCCN1CCCC1.OC=1C=CC2=C(NC(CO2)=O)C1>>COC=1C=C2C(=NC=NC2=CC1OCCCN1CCCC1)OC=1C=CC2=C(NC(CO2)=O)C1
Cl[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:24]([O:25][CH2:26][CH2:27][CH2:28][N:29]3[CH2:30][CH2:31][CH2:32][CH2:33]3)[cH:23][c:22]2[n:21][cH:20][n:19]1.[OH:7][c:8]1[cH:9][cH:10][c:11]2[c:12]([cH:13]1)[NH:14][C:15](=[O:16])[CH2:17][O:18]2>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([O:7][c:8]3[cH:9][cH:10][c:11]4[c:12]([cH:13]...
COc1cc2c(Cl)ncnc2cc1OCCCN1CCCC1.O=C1COc2ccc(O)cc2N1
COc1cc2c(Oc3ccc4c(c3)NC(=O)CO4)ncnc2cc1OCCCN1CCCC1
null
null
null
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
2d25b59c80a437134e7830160726da4e12ee4089c37759035843c1cccd8cd262
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
O=C1COc2ccc(Oc3ncnc4cc(OCCCN5CCCC5)ccc34)cc2N1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[OH;D1;+0:9]-[c:10](:[c:11]):[c:12]>>[c:11]:[c:10](-[O;H0;D2;+0:9]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8]):[c:12]
94.3
[{"value": 94.0, "product": "COC=1C=C2C(=NC=NC2=CC1OCCCN1CCCC1)OC=1C=CC2=C(NC(CO2)=O)C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 94.3, "product": "COC=1C=C2C(=NC=NC2=CC1OCCCN1CCCC1)OC=1C=CC2=C(NC(CO2)=O)C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Using a procedure analogous to that described for Example 9, 4-chloro-6-methoxy-7-(3-(pyrrolidin-1-yl)propoxy)quinazoline (0.13 g, 0.4 mmol), (prepared as described for the (starting material in Example 9), was reacted with 6-hydroxy-2H-4H-1,4-benzoxazin-3-one (83 mg, 0.5 mmol), (J. Chem. Soc. C, 1971, 2696), to give 6...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2c(c1)NCCO2.c1ccc2ncncc2c1.C1CC[NH]C1
HCl
null
null
null
COc1cc2c(Cl)ncnc2cc1OCCCN1CCCC1.O=C1COc2ccc(O)cc2N1>>COc1cc2c(Oc3ccc4c(c3)NC(=O)CO4)ncnc2cc1OCCCN1CCCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0529c424f3af499ab2e54e6225574c9a
COc1cc2c(Cl)ncnc2cc1OCC1CCN(C)CC1.Oc1ccc2ncccc2c1>>COc1cc2c(Oc3ccc4ncccc4c3)ncnc2cc1OCC1CCN(C)CC1
ClC1=NC=NC2=CC(=C(C=C12)OC)OCC1CCN(CC1)C.OC=1C=C2C=CC=NC2=CC1>>COC=1C=C2C(=NC=NC2=CC1OCC1CCN(CC1)C)OC=1C=C2C=CC=NC2=CC1
Cl[c:6]1[c:5]2[cH:4][c:3]([O:2][CH3:1])[c:23]([O:24][CH2:25][CH:26]3[CH2:27][CH2:28][N:29]([CH3:30])[CH2:31][CH2:32]3)[cH:22][c:21]2[n:20][cH:19][n:18]1.[OH:7][c:8]1[cH:9][cH:10][c:11]2[n:12][cH:13][cH:14][cH:15][c:16]2[cH:17]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]2[c:6]([O:7][c:8]3[cH:9][cH:10][c:11]4[n:12][cH:13][cH:14][cH:...
COc1cc2c(Cl)ncnc2cc1OCC1CCN(C)CC1.Oc1ccc2ncccc2c1
COc1cc2c(Oc3ccc4ncccc4c3)ncnc2cc1OCC1CCN(C)CC1
null
null
null
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
2d25b59c80a437134e7830160726da4e12ee4089c37759035843c1cccd8cd262
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1cnc2ccc(Oc3ncnc4cc(OCC5CCNCC5)ccc34)cc2c1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8].[OH;D1;+0:9]-[c:10](:[c:11]):[c:12]>>[c:11]:[c:10](-[O;H0;D2;+0:9]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[#7;a:4]:[c:5](:[c:6]):[c:7]:1:[c:8]):[c:12]
94
[{"value": 94.0, "product": "COC=1C=C2C(=NC=NC2=CC1OCC1CCN(CC1)C)OC=1C=C2C=CC=NC2=CC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 89.9, "product": "COC=1C=C2C(=NC=NC2=CC1OCC1CCN(CC1)C)OC=1C=C2C=CC=NC2=CC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Using a procedure analogous to that described for Example 10, 4-chloro-6-methoxy-7-((1-methylpiperidin-4-yl)methoxy)quinazoline (74 mg, 0.23 mmol), (prepared as described for the starting material in Example 10), was reacted with 6-hydroxyquinoline (41 mg, 0.28 mol) to give 6-methoxy-7-((1-methylpiperidin-4-yl)methoxy)...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1ccc2ncncc2c1
c1ccc2ncncc2c1
c1ccc2ncccc2c1.c1ccc2ncncc2c1.C1CC[NH]CC1
HCl
null
null
null
COc1cc2c(Cl)ncnc2cc1OCC1CCN(C)CC1.Oc1ccc2ncccc2c1>>COc1cc2c(Oc3ccc4ncccc4c3)ncnc2cc1OCC1CCN(C)CC1