dataset_id
large_stringclasses
414 values
reaction_id
large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
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large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-2d0a2336539b45ccbf1ab591a226384a
CC#CCn1c(Cl)nc2c1c(=O)n(CCc1ccccc1)c(=O)n2CC(=O)OCC.CC(C)(C)OC(=O)N1CCNCC1>>CC#CCn1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(CCc1ccccc1)c(=O)n2CC(=O)OCC
C(C)OC(CN1C(N(C(C=2N(C(=NC12)Cl)CC#CC)=O)CCC1=CC=CC=C1)=O)=O.C(C)(C)(C)OC(=O)N1CCNCC1>>C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2N(C(N(C(C2N1CC#CC)=O)CCC1=CC=CC=C1)=O)CC(=O)OCC
Cl[c:6]1[n:5]([CH2:4][C:3]#[C:2][CH3:1])[c:22]2[c:21]([n:20]1)[n:36]([CH2:37][C:38](=[O:39])[O:40][CH2:41][CH3:42])[c:34](=[O:35])[n:25]([CH2:26][CH2:27][c:28]1[cH:29][cH:30][cH:31][cH:32][cH:33]1)[c:23]2=[O:24].[NH:7]1[CH2:8][CH2:9][N:10]([C:11](=[O:12])[O:13][C:14]([CH3:15])([CH3:16])[CH3:17])[CH2:18][CH2:19]1>>[CH3:...
CC#CCn1c(Cl)nc2c1c(=O)n(CCc1ccccc1)c(=O)n2CC(=O)OCC.CC(C)(C)OC(=O)N1CCNCC1
CC#CCn1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(CCc1ccccc1)c(=O)n2CC(=O)OCC
null
null
null
Heteroatom Alkylation and Arylation
Ullmann-Goldberg Substitution amine
e5786cd15d554d1321f1795004da6d6c939bb0ddb133e8fc80dccdf8a8a64c61
b6b8e2cdb45054a35f5e8157d624f852c0601a09401556706e166b19536eb7a7
O=c1[nH]c2nc(N3CCNCC3)[nH]c2c(=O)n1CCc1ccccc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](:[#7;a:4]):[c:5](:[c:6]:[#7;a:7]):[#7;a:8]:1-[C:9]-[C:10]#[C:11].[#7:12]1-[C:13]-[C:14]-[NH;D2;+0:15]-[C:16]-[C:17]-1>>[#7;a:7]:[c:6]:[c:5]1:[#7;a:8](-[C:9]-[C:10]#[C:11]):[c;H0;D3;+0:1](-[N;H0;D3;+0:15]2-[C:14]-[C:13]-[#7:12]-[C:17]-[C:16]-2):[#7;a:2]:[c:3]:1:[#7;a:4]
86.9
[{"value": 86.9, "product": "C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2N(C(N(C(C2N1CC#CC)=O)CCC1=CC=CC=C1)=O)CC(=O)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
150
CELSIUS
null
null
A mixture of [7-(2-butynyl)-8-chloro-1-(2-phenylethyl)-2,6-dioxo-1,2,6,7-tetrahydropurin-3-yl]acetic acid ethyl ester (273 mg) and piperazine-1-carboxylic acid tert-butyl ester (360 mg) was heated in an oil bath of 150° C. for 30 minutes. The reaction mixture was purified by silica gel column chromatography using 20–30...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Secondary amine
Tertiary amine
c1ncc2[nH]cnc2n1.C1CNCC[NH]1
C1C[NH]CC[NH]1.c1ncc2[nH]cnc2n1
C1C[NH]CC[NH]1.c1ncc2[nH]cnc2n1.c1ccccc1
HCl
null
150
null
CC#CCn1c(Cl)nc2c1c(=O)n(CCc1ccccc1)c(=O)n2CC(=O)OCC.CC(C)(C)OC(=O)N1CCNCC1>>CC#CCn1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(CCc1ccccc1)c(=O)n2CC(=O)OCC
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-8ae045dfb96b445facc711999bb05522
CC#CCn1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(CCc1ccccc1)c(=O)n2CC(=O)OCC>>CC#CCn1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(CCc1ccccc1)c(=O)n2CC(=O)O
Cl.C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2N(C(N(C(C2N1CC#CC)=O)CCC1=CC=CC=C1)=O)CC(=O)OCC.[OH-].[Na+]>>C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2N(C(N(C(C2N1CC#CC)=O)CCC1=CC=CC=C1)=O)CC(=O)O
CC[O:40][C:38]([CH2:37][n:36]1[c:21]2[n:20][c:6]([N:7]3[CH2:8][CH2:9][N:10]([C:11](=[O:12])[O:13][C:14]([CH3:15])([CH3:16])[CH3:17])[CH2:18][CH2:19]3)[n:5]([CH2:4][C:3]#[C:2][CH3:1])[c:22]2[c:23](=[O:24])[n:25]([CH2:26][CH2:27][c:28]2[cH:29][cH:30][cH:31][cH:32][cH:33]2)[c:34]1=[O:35])=[O:39]>>[CH3:1][C:2]#[C:3][CH2:4]...
CC#CCn1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(CCc1ccccc1)c(=O)n2CC(=O)OCC
CC#CCn1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(CCc1ccccc1)c(=O)n2CC(=O)O
null
null
C(C)O
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=c1[nH]c2nc(N3CCNCC3)[nH]c2c(=O)n1CCc1ccccc1
C-C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
91.8
[{"value": 91.8, "product": "C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2N(C(N(C(C2N1CC#CC)=O)CCC1=CC=CC=C1)=O)CC(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
50
CELSIUS
null
null
A mixture of 4-[7-(2-butynyl)-3-ethoxycarbonylmethyl-1-(2-phenylethyl)-2,6-dioxo-1,2,6,7-tetrahydropurin-8-yl]piperazine-1-carboxylic acid tert-butyl ester (190 mg), ethanol (3 ml), and 1N aqueous sodium hydroxide solution (0.5 ml) was stirred with heating in an oil bath of 50° C. for 2 hours. 1N aqueous hydrochloric a...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
C1C[NH]CC[NH]1.c1ncc2[nH]cnc2n1.c1ccccc1
Other
C(C)O
50
null
CC#CCn1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(CCc1ccccc1)c(=O)n2CC(=O)OCC>C(C)O>CC#CCn1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(CCc1ccccc1)c(=O)n2CC(=O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-05af923f27e44bcd82fbacfe45c061f1
CC#CCn1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(CCN=[N+]=[N-])c(=O)n2C>>CC#CCn1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(CCN)c(=O)n2C
C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2N(C(N(C(C2N1CC#CC)=O)CCN=[N+]=[N-])=O)C.O.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1>>C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2N(C(N(C(C2N1CC#CC)=O)CCN)=O)C
[N-]=[N+]=[N:28][CH2:27][CH2:26][n:25]1[c:23](=[O:24])[c:22]2[n:5]([CH2:4][C:3]#[C:2][CH3:1])[c:6]([N:7]3[CH2:8][CH2:9][N:10]([C:11](=[O:12])[O:13][C:14]([CH3:15])([CH3:16])[CH3:17])[CH2:18][CH2:19]3)[n:20][c:21]2[n:31]([CH3:32])[c:29]1=[O:30]>>[CH3:1][C:2]#[C:3][CH2:4][n:5]1[c:6]([N:7]2[CH2:8][CH2:9][N:10]([C:11](=[O:...
CC#CCn1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(CCN=[N+]=[N-])c(=O)n2C
CC#CCn1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(CCN)c(=O)n2C
null
null
O1CCCC1
Reduction
Azide to amine reduction (Staudinger)
4c9e4990dae2bb965dec06bd45e318560989ee3681b61e443f7aa363b7cfa222
cd009d687d606bf351eac9390a176d16be38f2c8216a599b398641009c215027
O=c1[nH]c(=O)c2[nH]c(N3CCNCC3)nc2[nH]1
[C:1]-[C:2]-[N;H0;D2;+0:3]=[N+]=[N-]>>[C:1]-[C:2]-[NH2;D1;+0:3]
74.7
[{"value": 74.7, "product": "C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2N(C(N(C(C2N1CC#CC)=O)CCN)=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
4-[1-(2-Azidoethyl)-7-(2-butynyl)-3-methyl-2,6-dioxo-2,3,6,7-tetrahydro-1H-purin-8-yl]piperazine-1-carboxylic acid tert-butyl ester (0.17 g) was dissolved in tetrahydrofuran (3.5 ml), and water (0.23 ml) and triphenylphosphine (0.13 g) were added to the solution. After the mixture was stirred at room temperature overni...
10.6084/m9.figshare.5104873.v1
null
Azide
Primary amine
null
null
C1C[NH]CC[NH]1.c1ncc2[nH]cnc2n1
Other
O1CCCC1
null
8
CC#CCn1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(CCN=[N+]=[N-])c(=O)n2C>O1CCCC1>CC#CCn1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(CCN)c(=O)n2C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-469fd5b0efd24e2eb3d5f6ee45439c61
CI.Cn1c(=O)c2c(ncn2-c2ccccc2C(O)C2CN(C(=O)OC(C)(C)C)CCN2C(=O)OC(C)(C)C)n(C)c1=O.S=C=S>>CSC(=S)OC(c1ccccc1-n1cnc2c1c(=O)n(C)c(=O)n2C)C1CN(C(=O)OC(C)(C)C)CCN1C(=O)OC(C)(C)C
CI.[H-].[Na+].C(C)(C)(C)OC(=O)N1C(CN(CC1)C(=O)OC(C)(C)C)C(O)C1=C(C=CC=C1)N1C=NC=2N(C(N(C(C12)=O)C)=O)C.C(=S)=S>>C(C)(C)(C)OC(=O)N1C(CN(CC1)C(=O)OC(C)(C)C)C(OC(=S)SC)C1=C(C=CC=C1)N1C=NC=2N(C(N(C(C12)=O)C)=O)C
I[CH3:1].[OH:5][CH:6]([c:7]1[cH:8][cH:9][cH:10][cH:11][c:12]1-[n:13]1[cH:14][n:15][c:16]2[c:17]1[c:18](=[O:19])[n:20]([CH3:21])[c:22](=[O:23])[n:24]2[CH3:25])[CH:26]1[CH2:27][N:28]([C:29](=[O:30])[O:31][C:32]([CH3:33])([CH3:34])[CH3:35])[CH2:36][CH2:37][N:38]1[C:39](=[O:40])[O:41][C:42]([CH3:43])([CH3:44])[CH3:45].[S:2...
CI.Cn1c(=O)c2c(ncn2-c2ccccc2C(O)C2CN(C(=O)OC(C)(C)C)CCN2C(=O)OC(C)(C)C)n(C)c1=O.S=C=S
CSC(=S)OC(c1ccccc1-n1cnc2c1c(=O)n(C)c(=O)n2C)C1CN(C(=O)OC(C)(C)C)CCN1C(=O)OC(C)(C)C
null
null
O1CCCC1.O.C(C)(=O)OCC
Acylation
OtherReaction
c7dbbaabeba4030ac13d21dbea2d065e6ae27d66135e28ce4afa6269505c204f
8561a960f931e5a14f0c8246c71006c703df6abcd58e014f5406ceb13cbbe0b8
O=c1[nH]c(=O)c2c(ncn2-c2ccccc2CC2CNCCN2)[nH]1
I-[CH3;D1;+0:1].[#7:2]-[C:3]-[C:4](-[OH;D1;+0:5])-[c:6].[S;D1;H0:7]=[C;H0;D2;+0:8]=[S;H0;D1;+0:9]>>[#7:2]-[C:3]-[C:4](-[c:6])-[O;H0;D2;+0:5]-[C;H0;D3;+0:8](=[S;D1;H0:7])-[S;H0;D2;+0:9]-[CH3;D1;+0:1]
null
[]
null
null
20
MINUTE
Sodium hydride (60% oleaginous) was added to a solution of 2-[[2-(1,3-dimethyl-2,6-dioxo-1,2,3,6-tetrahydropurin-7-yl)-phenyl]hydroxymethyl]piperazine-1,4-dicarboxylic acid di-tert-butyl ester (low polarity) (0.214 g) in tetrahydrofuran (10 ml) at 0° C. under nitrogen atmosphere, and the mixture was stirred at room tem...
10.6084/m9.figshare.5104873.v1
null
Secondary alcohol
Ether.Thiocarbonyl.Monosulfide
null
null
c1ccccc1.c1ncc2[nH]cnc2n1.C1C[NH]CC[NH]1
HI
O1CCCC1.O.C(C)(=O)OCC
null
0.333333
CI.Cn1c(=O)c2c(ncn2-c2ccccc2C(O)C2CN(C(=O)OC(C)(C)C)CCN2C(=O)OC(C)(C)C)n(C)c1=O.S=C=S>O1CCCC1.O.C(C)(=O)OCC>CSC(=S)OC(c1ccccc1-n1cnc2c1c(=O)n(C)c(=O)n2C)C1CN(C(=O)OC(C)(C)C)CCN1C(=O)OC(C)(C)C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-16033799dbbf4bf0af540394b12d32de
CSC(=S)OC(c1ccccc1-n1cnc2c1c(=O)n(C)c(=O)n2C)C1CN(C(=O)OC(C)(C)C)CCN1C(=O)OC(C)(C)C>>Cn1c(=O)c2c(ncn2-c2ccccc2CC2CN(C(=O)OC(C)(C)C)CCN2C(=O)OC(C)(C)C)n(C)c1=O
C(C)(C)(C)OC(=O)N1C(CN(CC1)C(=O)OC(C)(C)C)C(OC(=S)SC)C1=C(C=CC=C1)N1C=NC=2N(C(N(C(C12)=O)C)=O)C.C(CCC)[SnH](CCCC)CCCC.N(=NC(C#N)(C)C)C(C#N)(C)C>>C(C)(C)(C)OC(=O)N1C(CN(CC1)C(=O)OC(C)(C)C)CC1=C(C=CC=C1)N1C=NC=2N(C(N(C(C12)=O)C)=O)C
CSC(=S)O[CH:16]([c:15]1[c:10](-[n:9]2[c:5]3[c:3](=[O:4])[n:2]([CH3:1])[c:39](=[O:40])[n:37]([CH3:38])[c:6]3[n:7][cH:8]2)[cH:11][cH:12][cH:13][cH:14]1)[CH:17]1[CH2:18][N:19]([C:20](=[O:21])[O:22][C:23]([CH3:24])([CH3:25])[CH3:26])[CH2:27][CH2:28][N:29]1[C:30](=[O:31])[O:32][C:33]([CH3:34])([CH3:35])[CH3:36]>>[CH3:1][n:2...
CSC(=S)OC(c1ccccc1-n1cnc2c1c(=O)n(C)c(=O)n2C)C1CN(C(=O)OC(C)(C)C)CCN1C(=O)OC(C)(C)C
Cn1c(=O)c2c(ncn2-c2ccccc2CC2CN(C(=O)OC(C)(C)C)CCN2C(=O)OC(C)(C)C)n(C)c1=O
null
null
C1(=CC=CC=C1)C
Reduction
OtherReaction
4a66c27853427274b272243a753c9056b0872c3b53082a3e92fbfe42b48d2aca
b7a5234770726d9df7bf8a7a8600249246518d52f4a289b48469a444ad416279
O=c1[nH]c(=O)c2c(ncn2-c2ccccc2CC2CNCCN2)[nH]1
C-S-C(=S)-O-[CH;D3;+0:1](-[C:2](-[C:3]-[#7:4])-[#7:5](-[C:6](=[O;D1;H0:7])-[#8:8]-[C:9](-[C;D1;H3:10])(-[C;D1;H3:11])-[C;D1;H3:12])-[C:13])-[c:14](:[c:15]):[c:16]>>[#7:4]-[C:3]-[C:2](-[CH2;D2;+0:1]-[c:14](:[c:15]):[c:16])-[#7:5](-[C:6](=[O;D1;H0:7])-[#8:8]-[C:9](-[C;D1;H3:10])(-[C;D1;H3:11])-[C;D1;H3:12])-[C:13]
83.7
[{"value": 83.7, "product": "C(C)(C)(C)OC(=O)N1C(CN(CC1)C(=O)OC(C)(C)C)CC1=C(C=CC=C1)N1C=NC=2N(C(N(C(C12)=O)C)=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
2-[1-[2-(1,3-Dimethyl-2,6-dioxo-1,2,3,6-tetrahydropurin-7-yl)-phenyl]-1-methylsulfanylthiocarbonyloxymethyl]piperazine-1,4-dicarboxylic acid di-tert-butyl ester (low polarity) (0.175 g), tributyltin hydride (0.25 g), and 2,2′-azobis(isobutyronitrile) (0.010 g) were dissolved in toluene (5 ml) under nitrogen atmosphere,...
10.6084/m9.figshare.5104873.v1
null
Ether.Thiocarbonyl.Monosulfide
null
null
null
c1ncc2nc[nH]c2n1.c1ccccc1.C1C[NH]CC[NH]1
Other
C1(=CC=CC=C1)C
null
null
CSC(=S)OC(c1ccccc1-n1cnc2c1c(=O)n(C)c(=O)n2C)C1CN(C(=O)OC(C)(C)C)CCN1C(=O)OC(C)(C)C>C1(=CC=CC=C1)C>Cn1c(=O)c2c(ncn2-c2ccccc2CC2CN(C(=O)OC(C)(C)C)CCN2C(=O)OC(C)(C)C)n(C)c1=O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ab99aab08c6b4fb0ae2b6f9fa5a52a16
Cn1c(=O)c2c(ncn2-c2ccccc2CC2CN(C(=O)OC(C)(C)C)CCN2C(=O)OC(C)(C)C)n(C)c1=O>>Cn1c(=O)c2c(nc3n2-c2ccccc2CC2CNCCN32)n(C)c1=O
C(C)(C)(C)OC(=O)N1C(CN(CC1)C(=O)OC(C)(C)C)CC1=C(C=CC=C1)N1C=NC=2N(C(N(C(C12)=O)C)=O)C.FC(C(=O)O)(F)F>>FC(C(=O)O)(F)F.CN1C(N(C(C2=C1N=C1N3C(CC4=C(N21)C=CC=C4)CNCC3)=O)C)=O
CC(C)(C)OC(=O)[N:19]1[CH2:18][CH:17]([CH2:16][c:15]2[c:10](-[n:9]3[c:5]4[c:3](=[O:4])[n:2]([CH3:1])[c:25](=[O:26])[n:23]([CH3:24])[c:6]4[n:7][cH:8]3)[cH:11][cH:12][cH:13][cH:14]2)[N:22](C(=O)OC(C)(C)C)[CH2:21][CH2:20]1>>[CH3:1][n:2]1[c:3](=[O:4])[c:5]2[c:6]([n:7][c:8]3[n:9]2-[c:10]2[cH:11][cH:12][cH:13][cH:14][c:15]2[C...
Cn1c(=O)c2c(ncn2-c2ccccc2CC2CN(C(=O)OC(C)(C)C)CCN2C(=O)OC(C)(C)C)n(C)c1=O
Cn1c(=O)c2c(nc3n2-c2ccccc2CC2CNCCN32)n(C)c1=O
null
null
null
Functional Group Interconversion
OtherReaction
603730c751d479d06b06dd4cfbe9ece0d6ac9b32e8c6c5a726ee664fb6aa9be1
98954e35dd97aa5fdb6b2d6cc2d26f8aaed3dcf612f871e78a8e228b88dc1fd5
O=c1[nH]c(=O)c2c(nc3n2-c2ccccc2CC2CNCCN32)[nH]1
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1]1-[C:2]-[C:3](-[C:4])-[N;H0;D3;+0:5](-C(=O)-O-C(-C)(-C)-C)-[C:6]-[C:7]-1.[C;D1;H3:8]-[#7;a:9]1:[c:10]:[#7;a:11]:[c:12]:[c:13]2:[#7;a:14](-[c:15]):[cH;D2;+0:16]:[#7;a:17]:[c:18]:1:2>>[C:4]-[C:3]1-[C:2]-[NH;D2;+0:1]-[C:7]-[C:6]-[N;H0;D3;+0:5]-1-[c;H0;D3;+0:16]1:[#7;a:17]:[c:18]2:[#7;a:9]...
null
[]
null
null
30
MINUTE
2-[2-(1,3-dimethyl-2,6-dioxo-1,2,3,6-tetrahydropurin-7-yl)benzyl]piperazine-1,4-dicarboxylic acid di-tert-butyl ester (0.055 g) was dissolved in trifluoroacetic acid (0.5 ml), the mixture was stirred for 30 minutes, and the solvent was removed by distillation at reduced pressure. The residue was dissolved in N,N-dimeth...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Carbamic ester.Ether.Ether.Boc.Boc
Secondary amine.Tertiary amine
C1C[NH]CC[NH]1.c1ncc2[nH]cnc2n1
c1ccc2c(c1)CC1CNCCN1c1nc3ncncc3n12
c1ccc2c(c1)CC1CNCCN1c1nc3ncncc3n12
HO-
null
null
0.5
Cn1c(=O)c2c(ncn2-c2ccccc2CC2CN(C(=O)OC(C)(C)C)CCN2C(=O)OC(C)(C)C)n(C)c1=O>>Cn1c(=O)c2c(nc3n2-c2ccccc2CC2CNCCN32)n(C)c1=O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-05e81e29142c4ae0868982a133fee016
CC(C)(C)C(=O)OCn1c(=O)c2[nH]cnc2n(COC(=O)C(C)(C)C)c1=O.O=Cc1ccccc1B(O)O>>CC(C)(C)C(=O)OCn1c(=O)c2c(ncn2-c2ccccc2C=O)n(COC(=O)C(C)(C)C)c1=O
CC(C(=O)OCN1C(N(C(C=2NC=NC12)=O)COC(C(C)(C)C)=O)=O)(C)C.C(=O)C1=C(C=CC=C1)B(O)O.N1=CC=CC=C1>>CC(C(=O)OCN1C(N(C=2N=CN(C2C1=O)C1=C(C=CC=C1)C=O)COC(C(C)(C)C)=O)=O)(C)C
[CH3:1][C:2]([CH3:3])([CH3:4])[C:5](=[O:6])[O:7][CH2:8][n:9]1[c:10](=[O:11])[c:12]2[c:13]([n:14][cH:15][nH:16]2)[n:25]([CH2:26][O:27][C:28](=[O:29])[C:30]([CH3:31])([CH3:32])[CH3:33])[c:34]1=[O:35].OB(O)[c:17]1[cH:18][cH:19][cH:20][cH:21][c:22]1[CH:23]=[O:24]>>[CH3:1][C:2]([CH3:3])([CH3:4])[C:5](=[O:6])[O:7][CH2:8][n:9...
CC(C)(C)C(=O)OCn1c(=O)c2[nH]cnc2n(COC(=O)C(C)(C)C)c1=O.O=Cc1ccccc1B(O)O
CC(C)(C)C(=O)OCn1c(=O)c2c(ncn2-c2ccccc2C=O)n(COC(=O)C(C)(C)C)c1=O
null
C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-]
CN(C=O)C.C(C)(=O)OCC
Heteroatom Alkylation and Arylation
OtherReaction
193a52be698a8cc7c00a0e51f250e81e1eef3fc7f6e6eee9787e052516f6fde7
e0368246531386f86cd0aa9da1423eb47f529b782fb229563cefe1166d6ba4f5
O=c1[nH]c(=O)c2c(ncn2-c2ccccc2)[nH]1
O-B(-O)-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[C:5]=[O;D1;H0:6]):[c:7].[C:8]-[#7;a:9]1:[c:10]:[#7;a:11](-[C:12]):[c:13](=[O;D1;H0:14]):[c:15]2:[nH;D2;+0:16]:[c:17]:[#7;a:18]:[c:19]:1:2>>[C:8]-[#7;a:9]1:[c:10]:[#7;a:11](-[C:12]):[c:13](=[O;D1;H0:14]):[c:15]2:[c:19]:1:[#7;a:18]:[c:17]:[n;H0;D3;+0:16]:2-[c;H0;D3;+0:1](:[c:2...
31.7
[{"value": 31.7, "product": "CC(C(=O)OCN1C(N(C=2N=CN(C2C1=O)C1=C(C=CC=C1)C=O)COC(C(C)(C)C)=O)=O)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
37
HOUR
2,2-Dimethylpropionic acid [3-(2,2-dimethylpropionyloxymethyl)-2,6-dioxo-2,3,6,7-tetrahydropurin-1-yl]methyl ester (10.2 g), 2-formylphenylboronic acid (8.04 g), and copper(II) acetate (7.30 g) were suspended in N,N-dimethylformamide (50 ml), pyridine (4.34 ml) was added thereto, and the mixture was stirred at room tem...
10.6084/m9.figshare.5104873.v1
null
Boronic acid
null
c1ncc2nc[nH]c2n1.c1ccccc1
c1ncc2nc[nH]c2n1.c1ccccc1
c1ncc2nc[nH]c2n1.c1ccccc1
HO-.B
C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-].CN(C=O)C.C(C)(=O)OCC
null
37
CC(C)(C)C(=O)OCn1c(=O)c2[nH]cnc2n(COC(=O)C(C)(C)C)c1=O.O=Cc1ccccc1B(O)O>C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-].CN(C=O)C.C(C)(=O)OCC>CC(C)(C)C(=O)OCn1c(=O)c2c(ncn2-c2ccccc2C=O)n(COC(=O)C(C)(C)C)c1=O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4827b0d3f5684e7292dc522efb21c879
CC(C)(C)C(=O)OCn1c(=O)c2c(ncn2-c2ccccc2C=O)n(COC(=O)C(C)(C)C)c1=O.O=C1CCC(=O)N1Cl>>CC(C)(C)C(=O)OCn1c(=O)c2c(nc(Cl)n2-c2ccccc2C=O)n(COC(=O)C(C)(C)C)c1=O
CC(C(=O)OCN1C(N(C=2N=CN(C2C1=O)C1=C(C=CC=C1)C=O)COC(C(C)(C)C)=O)=O)(C)C.ClN1C(CCC1=O)=O>>ClC1=NC=2N(C(N(C(C2N1C1=C(C=CC=C1)C=O)=O)COC(C(C)(C)C)=O)=O)COC(C(C)(C)C)=O
[CH3:1][C:2]([CH3:3])([CH3:4])[C:5](=[O:6])[O:7][CH2:8][n:9]1[c:10](=[O:11])[c:12]2[c:13]([n:14][cH:15][n:17]2-[c:18]2[cH:19][cH:20][cH:21][cH:22][c:23]2[CH:24]=[O:25])[n:26]([CH2:27][O:28][C:29](=[O:30])[C:31]([CH3:32])([CH3:33])[CH3:34])[c:35]1=[O:36].O=C1CCC(=O)N1[Cl:16]>>[CH3:1][C:2]([CH3:3])([CH3:4])[C:5](=[O:6])[...
CC(C)(C)C(=O)OCn1c(=O)c2c(ncn2-c2ccccc2C=O)n(COC(=O)C(C)(C)C)c1=O.O=C1CCC(=O)N1Cl
CC(C)(C)C(=O)OCn1c(=O)c2c(nc(Cl)n2-c2ccccc2C=O)n(COC(=O)C(C)(C)C)c1=O
null
null
CN(C=O)C.C(C)(=O)OCC
Functional Group Interconversion
Chlorination
14c81eccfe7222df9f154a6d36de877a8f4fe32e30972af529ae83dcf968a138
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
O=c1[nH]c(=O)c2c(ncn2-c2ccccc2)[nH]1
O=C1-C-C-C(=O)-N-1-[Cl;H0;D1;+0:1].[#7;a:2]:[c:3]1:[#7;a:4]:[cH;D2;+0:5]:[#7;a:6](-[c:7]):[c:8]:1:[c:9]:[#7;a:10]>>[#7;a:2]:[c:3]1:[#7;a:4]:[c;H0;D3;+0:5](-[Cl;H0;D1;+0:1]):[#7;a:6](-[c:7]):[c:8]:1:[c:9]:[#7;a:10]
74.7
[{"value": 74.7, "product": "ClC1=NC=2N(C(N(C(C2N1C1=C(C=CC=C1)C=O)=O)COC(C(C)(C)C)=O)=O)COC(C(C)(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
2,2-Dimethylpropionic acid [1-(2,2-dimethylpropionyloxymethyl)-7-(2-formylphenyl)-2,6-dioxo-1,2,6,7-tetrahydropurin-3-yl]methyl ester (2.50 g) and N-chlorosuccinimide (896 mg) were dissolved in N,N-dimethylformamide (25 ml), and the mixture was stirred at room temperature for 8 hours. The reaction mixture was diluted w...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1ncc2nc[nH]c2n1.C1CCNC1
c1ncc2nc[nH]c2n1
c1ncc2nc[nH]c2n1.c1ccccc1
HO-
CN(C=O)C.C(C)(=O)OCC
null
8
CC(C)(C)C(=O)OCn1c(=O)c2c(ncn2-c2ccccc2C=O)n(COC(=O)C(C)(C)C)c1=O.O=C1CCC(=O)N1Cl>CN(C=O)C.C(C)(=O)OCC>CC(C)(C)C(=O)OCn1c(=O)c2c(nc(Cl)n2-c2ccccc2C=O)n(COC(=O)C(C)(C)C)c1=O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-15d6af6873dd481bba186ab0b176bf15
CC(C)(C)C(=O)OCn1c(=O)c2c(nc(Cl)n2-c2ccccc2C=O)n(COC(=O)C(C)(C)C)c1=O.CC(C)(C)OC(=O)N1CCNCC1>>CC(C)(C)OC(=O)N1CCN(c2nc3c(c(=O)n(COC(=O)C(C)(C)C)c(=O)n3COC(=O)C(C)(C)C)n2-c2ccccc2C=O)CC1
ClC1=NC=2N(C(N(C(C2N1C1=C(C=CC=C1)C=O)=O)COC(C(C)(C)C)=O)=O)COC(C(C)(C)C)=O.C(C)(C)(C)OC(=O)N1CCNCC1>>C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2N(C(N(C(C2N1C1=C(C=CC=C1)C=O)=O)COC(C(C)(C)C)=O)=O)COC(C(C)(C)C)=O
Cl[c:12]1[n:13][c:14]2[c:15]([c:16](=[O:17])[n:18]([CH2:19][O:20][C:21](=[O:22])[C:23]([CH3:24])([CH3:25])[CH3:26])[c:27](=[O:28])[n:29]2[CH2:30][O:31][C:32](=[O:33])[C:34]([CH3:35])([CH3:36])[CH3:37])[n:38]1-[c:39]1[cH:40][cH:41][cH:42][cH:43][c:44]1[CH:45]=[O:46].[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[N:8]1...
CC(C)(C)C(=O)OCn1c(=O)c2c(nc(Cl)n2-c2ccccc2C=O)n(COC(=O)C(C)(C)C)c1=O.CC(C)(C)OC(=O)N1CCNCC1
CC(C)(C)OC(=O)N1CCN(c2nc3c(c(=O)n(COC(=O)C(C)(C)C)c(=O)n3COC(=O)C(C)(C)C)n2-c2ccccc2C=O)CC1
null
null
C(Cl)(Cl)Cl
Heteroatom Alkylation and Arylation
Ullmann-Goldberg Substitution amine
e9344fb5b31533e2c38d57778c7c82c0aa2d752545a4dd76e010d9a664cd15dc
b6b8e2cdb45054a35f5e8157d624f852c0601a09401556706e166b19536eb7a7
O=c1[nH]c(=O)c2c(nc(N3CCNCC3)n2-c2ccccc2)[nH]1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](:[#7;a:4]):[c:5](:[c:6]:[#7;a:7]):[#7;a:8]:1-[c:9].[#7:10]1-[C:11]-[C:12]-[NH;D2;+0:13]-[C:14]-[C:15]-1>>[#7;a:7]:[c:6]:[c:5]1:[#7;a:8](-[c:9]):[c;H0;D3;+0:1](-[N;H0;D3;+0:13]2-[C:14]-[C:15]-[#7:10]-[C:11]-[C:12]-2):[#7;a:2]:[c:3]:1:[#7;a:4]
75.3
[{"value": 75.3, "product": "C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2N(C(N(C(C2N1C1=C(C=CC=C1)C=O)=O)COC(C(C)(C)C)=O)=O)COC(C(C)(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
150
CELSIUS
10
MINUTE
2,2-Dimethylpropionic acid [8-chloro-1-(2,2-dimethyl-propionyloxymethyl)-7-(2-formylphenyl)-2,6-dioxo-1,2,6,7-tetrahydropurin-3-yl]methyl ester (2.0 g) and piperazine-1-carboxylic acid tert-butyl ester (2.15 g) were mixed, and the mixture was stirred at 150° C. for 1 hour and 10 minutes. The reaction mixture was dilute...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Secondary amine
Tertiary amine
c1ncc2nc[nH]c2n1.C1C[NH]CCN1
C1C[NH]CC[NH]1.c1ncc2nc[nH]c2n1
C1C[NH]CC[NH]1.c1ncc2nc[nH]c2n1.c1ccccc1
HCl
C(Cl)(Cl)Cl
150
0.166667
CC(C)(C)C(=O)OCn1c(=O)c2c(nc(Cl)n2-c2ccccc2C=O)n(COC(=O)C(C)(C)C)c1=O.CC(C)(C)OC(=O)N1CCNCC1>C(Cl)(Cl)Cl>CC(C)(C)OC(=O)N1CCN(c2nc3c(c(=O)n(COC(=O)C(C)(C)C)c(=O)n3COC(=O)C(C)(C)C)n2-c2ccccc2C=O)CC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-43a4a930cbcd4fe4bd46bc76aade3211
CC(C)(C)OC(=O)N1CCN(c2nc3c(c(=O)n(COC(=O)C(C)(C)C)c(=O)n3COC(=O)C(C)(C)C)n2-c2ccccc2C=O)CC1>>C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(COC(=O)C(C)(C)C)c(=O)n2COC(=O)C(C)(C)C
O1CCCC1.CC(C)([O-])C.[K+].C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2N(C(N(C(C2N1C1=C(C=CC=C1)C=O)=O)COC(C(C)(C)C)=O)=O)COC(C(C)(C)C)=O.O1CCCC1>>C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2N(C(N(C(C2N1C1=C(C=CC=C1)C=C)=O)COC(C(C)(C)C)=O)=O)COC(C(C)(C)C)=O
O=[CH:2][c:3]1[cH:4][cH:5][cH:6][cH:7][c:8]1-[n:9]1[c:10]([N:11]2[CH2:12][CH2:13][N:14]([C:15](=[O:16])[O:17][C:18]([CH3:19])([CH3:20])[CH3:21])[CH2:22][CH2:23]2)[n:24][c:25]2[c:26]1[c:27](=[O:28])[n:29]([CH2:30][O:31][C:32](=[O:33])[C:34]([CH3:35])([CH3:36])[CH3:37])[c:38](=[O:39])[n:40]2[CH2:41][O:42][C:43](=[O:44])[...
CC(C)(C)OC(=O)N1CCN(c2nc3c(c(=O)n(COC(=O)C(C)(C)C)c(=O)n3COC(=O)C(C)(C)C)n2-c2ccccc2C=O)CC1
C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(COC(=O)C(C)(C)C)c(=O)n2COC(=O)C(C)(C)C
null
[Br-].C[P+](C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1
C(C)(=O)OCC
Functional Group Interconversion
OtherReaction
dd6fb167b4e71f3ea190d18ad4e87d18c641d879b83b47beb9dc06bc791584b1
6b3ec9b506a5bb4882685e77a1e07fcb518f891061dfbc2d36767289330c841e
O=c1[nH]c(=O)c2c(nc(N3CCNCC3)n2-c2ccccc2)[nH]1
O=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4]>>[C;D1;H2:5]=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
1
HOUR
Methyltriphenylphosphonium bromide (3.52 g) was dissolved in tetrahydrofuran (20 ml), potassium tert-butoxide (948 mg) was added to the solution, and the mixture was stirred at room temperature for 1 hour. A solution of 4-[1,3-bis(2,2-dimethylpropionyloxymethyl)-7-(2-formylphenyl)-2,6-dioxo-2,3,6,7-tetrahydro-1H-purin-...
10.6084/m9.figshare.5104873.v1
null
Aldehyde
Vinyl
null
null
c1ccccc1.C1C[NH]CC[NH]1.c1ncc2[nH]cnc2n1
null
[Br-].C[P+](C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1.C(C)(=O)OCC
null
1
CC(C)(C)OC(=O)N1CCN(c2nc3c(c(=O)n(COC(=O)C(C)(C)C)c(=O)n3COC(=O)C(C)(C)C)n2-c2ccccc2C=O)CC1>[Br-].C[P+](C1=CC=CC=C1)(C1=CC=CC=C1)C1=CC=CC=C1.C(C)(=O)OCC>C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(COC(=O)C(C)(C)C)c(=O)n2COC(=O)C(C)(C)C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-dbb5d32f258e4e769350aaf68d59b9a5
C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(COC(=O)C(C)(C)C)c(=O)n2COC(=O)C(C)(C)C>>C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2[nH]c(=O)n(COC(=O)C(C)(C)C)c(=O)c21
[H-].[Na+].C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2N(C(N(C(C2N1C1=C(C=CC=C1)C=C)=O)COC(C(C)(C)C)=O)=O)COC(C(C)(C)C)=O>>C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2NC(N(C(C2N1C1=C(C=CC=C1)C=C)=O)COC(C(C)(C)C)=O)=O
CC(C)(C)C(=O)OC[n:26]1[c:25]2[n:24][c:10]([N:11]3[CH2:12][CH2:13][N:14]([C:15](=[O:16])[O:17][C:18]([CH3:19])([CH3:20])[CH3:21])[CH2:22][CH2:23]3)[n:9](-[c:8]3[c:3]([CH:2]=[CH2:1])[cH:4][cH:5][cH:6][cH:7]3)[c:40]2[c:38](=[O:39])[n:29]([CH2:30][O:31][C:32](=[O:33])[C:34]([CH3:35])([CH3:36])[CH3:37])[c:27]1=[O:28]>>[CH2:...
C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(COC(=O)C(C)(C)C)c(=O)n2COC(=O)C(C)(C)C
C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2[nH]c(=O)n(COC(=O)C(C)(C)C)c(=O)c21
null
null
O1CCCC1.C(Cl)(Cl)Cl.CO
Reduction
OtherReaction
640a644854d0d424f3b2f603152cc1a7aea1cadf590f863f6706eb0b62b24502
b8e5da8ea19c403a2e974791a9cf591400749acb6b71151717aaece4f3b22bef
O=c1[nH]c(=O)c2c(nc(N3CCNCC3)n2-c2ccccc2)[nH]1
C-C(-C)(-C)-C(=O)-O-C-[n;H0;D3;+0:1]1:[c:2]2:[#7;a:3]:[c:4]:[#7;a:5](-[c:6]):[c:7]:2:[c:8]:[#7;a:9](-[C:10]):[c:11]:1=[O;D1;H0:12]>>[C:10]-[#7;a:9]1:[c:8]:[c:7]2:[#7;a:5](-[c:6]):[c:4]:[#7;a:3]:[c:2]:2:[nH;D2;+0:1]:[c:11]:1=[O;D1;H0:12]
87.4
[{"value": 87.4, "product": "C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2NC(N(C(C2N1C1=C(C=CC=C1)C=C)=O)COC(C(C)(C)C)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
17
MINUTE
4-[1,3-Bis(2,2-dimethylpropionyloxymethyl)-2,6-dioxo-7-(2-vinylphenyl)-2,3,6,7-tetrahydro-1H-purin-8-yl]piperazine-1-carboxylic acid tert-butyl ester (704 mg) was dissolved in tetrahydrofuran (7 ml) and methanol (14 ml), sodium hydride (51 mg) was added to the solution, and the mixture was stirred at room temperature f...
10.6084/m9.figshare.5104873.v1
null
Ester
null
c1ncc2nc[nH]c2n1
c1ncc2[nH]cnc2n1
c1ccccc1.C1C[NH]CC[NH]1.c1ncc2[nH]cnc2n1
HO-
O1CCCC1.C(Cl)(Cl)Cl.CO
null
0.283333
C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(COC(=O)C(C)(C)C)c(=O)n2COC(=O)C(C)(C)C>O1CCCC1.C(Cl)(Cl)Cl.CO>C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2[nH]c(=O)n(COC(=O)C(C)(C)C)c(=O)c21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-adf3dc29b84349008f1bd7593bcf1b04
C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2[nH]c(=O)n(COC(=O)C(C)(C)C)c(=O)c21.CCOC(=O)CBr>>C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(COC(=O)C(C)(C)C)c(=O)n2CC(=O)OCC
C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2NC(N(C(C2N1C1=C(C=CC=C1)C=C)=O)COC(C(C)(C)C)=O)=O.BrCC(=O)OCC.C([O-])([O-])=O.[K+].[K+]>>C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2N(C(N(C(C2N1C1=C(C=CC=C1)C=C)=O)COC(C(C)(C)C)=O)=O)CC(=O)OCC
[CH2:1]=[CH:2][c:3]1[cH:4][cH:5][cH:6][cH:7][c:8]1-[n:9]1[c:10]([N:11]2[CH2:12][CH2:13][N:14]([C:15](=[O:16])[O:17][C:18]([CH3:19])([CH3:20])[CH3:21])[CH2:22][CH2:23]2)[n:24][c:25]2[c:26]1[c:27](=[O:28])[n:29]([CH2:30][O:31][C:32](=[O:33])[C:34]([CH3:35])([CH3:36])[CH3:37])[c:38](=[O:39])[nH:40]2.Br[CH2:41][C:42](=[O:4...
C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2[nH]c(=O)n(COC(=O)C(C)(C)C)c(=O)c21.CCOC(=O)CBr
C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(COC(=O)C(C)(C)C)c(=O)n2CC(=O)OCC
null
null
CN(C=O)C.C(C)(=O)OCC
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
7d358008569a510febb7dbae9ae69699ebd741f56473500303ef0889f4be2b21
6007d70cc3173f3039a472489995dad2781e8d749be1f1aa209b0bf2f190a4b4
O=c1[nH]c(=O)c2c(nc(N3CCNCC3)n2-c2ccccc2)[nH]1
Br-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#8:4]-[C:5].[C:6]-[#7;a:7]1:[c:8]:[c:9]2:[#7;a:10](-[c:11]):[c:12]:[#7;a:13]:[c:14]:2:[nH;D2;+0:15]:[c:16]:1=[O;D1;H0:17]>>[C:6]-[#7;a:7]1:[c:8]:[c:9]2:[#7;a:10](-[c:11]):[c:12]:[#7;a:13]:[c:14]:2:[n;H0;D3;+0:15](-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#8:4]-[C:5]):[c:16]:1=[O;D1;H0:17...
null
[]
null
null
14
HOUR
4-[1-(2,2-Dimethylpropionyloxymethyl)-2,6-dioxo-7-(2-vinylphenyl)-2,3,6,7-tetrahydro-1H-purin-8-yl]piperazine-1-carboxylic acid tert-butyl ester (80 mg) was dissolved in N,N-dimethylformamide (2 ml), ethyl bromoacetate (19 μl) and potassium carbonate (22 mg) were added to the solution, and the mixture was stirred at ro...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester
Ester
c1ncc2[nH]cnc2n1
c1ncc2[nH]cnc2n1
c1ccccc1.C1C[NH]CC[NH]1.c1ncc2[nH]cnc2n1
HBr
CN(C=O)C.C(C)(=O)OCC
null
14
C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2[nH]c(=O)n(COC(=O)C(C)(C)C)c(=O)c21.CCOC(=O)CBr>CN(C=O)C.C(C)(=O)OCC>C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(COC(=O)C(C)(C)C)c(=O)n2CC(=O)OCC
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ea04dafa420d4f0d9abd859d79b64910
C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(COC(=O)C(C)(C)C)c(=O)n2CC(=O)OCC>>C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)[nH]c(=O)n2CC(=O)OCC
[H-].[Na+].C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2N(C(N(C(C2N1C1=C(C=CC=C1)C=C)=O)COC(C(C)(C)C)=O)=O)CC(=O)OCC>>C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2N(C(NC(C2N1C1=C(C=CC=C1)C=C)=O)=O)CC(=O)OCC
CC(C)(C)C(=O)OC[n:29]1[c:27](=[O:28])[c:26]2[n:9](-[c:8]3[c:3]([CH:2]=[CH2:1])[cH:4][cH:5][cH:6][cH:7]3)[c:10]([N:11]3[CH2:12][CH2:13][N:14]([C:15](=[O:16])[O:17][C:18]([CH3:19])([CH3:20])[CH3:21])[CH2:22][CH2:23]3)[n:24][c:25]2[n:32]([CH2:33][C:34](=[O:35])[O:36][CH2:37][CH3:38])[c:30]1=[O:31]>>[CH2:1]=[CH:2][c:3]1[cH...
C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(COC(=O)C(C)(C)C)c(=O)n2CC(=O)OCC
C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)[nH]c(=O)n2CC(=O)OCC
null
null
O1CCCC1.CO.C(C)(=O)OCC
Reduction
OtherReaction
df8a3c8b7aa7d10b48c9fb6d61e80538577be49615529cea0e9d9fc23715d092
b8e5da8ea19c403a2e974791a9cf591400749acb6b71151717aaece4f3b22bef
O=c1[nH]c(=O)c2c(nc(N3CCNCC3)n2-c2ccccc2)[nH]1
C-C(-C)(-C)-C(=O)-O-C-[n;H0;D3;+0:1]1:[c:2](=[O;D1;H0:3]):[c:4]2:[#7;a:5](-[c:6]):[c:7]:[#7;a:8]:[c:9]:2:[#7;a:10](-[C:11]-[C:12](-[#8:13])=[O;D1;H0:14]):[c:15]:1=[O;D1;H0:16]>>[#8:13]-[C:12](=[O;D1;H0:14])-[C:11]-[#7;a:10]1:[c:9]2:[#7;a:8]:[c:7]:[#7;a:5](-[c:6]):[c:4]:2:[c:2](=[O;D1;H0:3]):[nH;D2;+0:1]:[c:15]:1=[O;D1;...
82.1
[{"value": 82.1, "product": "C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2N(C(NC(C2N1C1=C(C=CC=C1)C=C)=O)=O)CC(=O)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3.5
HOUR
4-[1-(2,2-Dimethylpropionyloxymethyl)-3-ethoxycarbonylmethyl-2,6-dioxo-7-(2-vinylphenyl)-2,3,6,7-tetrahydro-1H-purin-8-yl]piperazine-1-carboxylic acid tert-butyl ester (89 mg) was dissolved in tetrahydrofuran (1 ml) and methanol (2 ml), sodium hydride (7 mg) was added to the solution, and the mixture was stirred at roo...
10.6084/m9.figshare.5104873.v1
null
Ester
null
c1ncc2[nH]cnc2n1
c1ncc2[nH]cnc2n1
c1ccccc1.C1C[NH]CC[NH]1.c1ncc2[nH]cnc2n1
HO-
O1CCCC1.CO.C(C)(=O)OCC
null
3.5
C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(COC(=O)C(C)(C)C)c(=O)n2CC(=O)OCC>O1CCCC1.CO.C(C)(=O)OCC>C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)[nH]c(=O)n2CC(=O)OCC
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-95e6c1ed76d642f8aca0012bb640c73c
C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)[nH]c(=O)n2CC(=O)OCC.CI>>C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(C)c(=O)n2CC(=O)OCC
C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2N(C(NC(C2N1C1=C(C=CC=C1)C=C)=O)=O)CC(=O)OCC.CI.C([O-])([O-])=O.[K+].[K+]>>C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2N(C(N(C(C2N1C1=C(C=CC=C1)C=C)=O)C)=O)CC(=O)OCC
[CH2:1]=[CH:2][c:3]1[cH:4][cH:5][cH:6][cH:7][c:8]1-[n:9]1[c:10]([N:11]2[CH2:12][CH2:13][N:14]([C:15](=[O:16])[O:17][C:18]([CH3:19])([CH3:20])[CH3:21])[CH2:22][CH2:23]2)[n:24][c:25]2[c:26]1[c:27](=[O:28])[nH:29][c:31](=[O:32])[n:33]2[CH2:34][C:35](=[O:36])[O:37][CH2:38][CH3:39].I[CH3:30]>>[CH2:1]=[CH:2][c:3]1[cH:4][cH:5...
C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)[nH]c(=O)n2CC(=O)OCC.CI
C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(C)c(=O)n2CC(=O)OCC
null
null
CN(C=O)C.C(C)(=O)OCC
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
011a6d20d1a2cde13aab96bd8efb9a0393d2f8a89a318e20bc7624b0300657a4
7a358c636daddc97c1fb4c29f378044d7eac3f01815d9966e599841f642d631a
O=c1[nH]c(=O)c2c(nc(N3CCNCC3)n2-c2ccccc2)[nH]1
I-[CH3;D1;+0:1].[#8:2]-[C:3](=[O;D1;H0:4])-[C:5]-[#7;a:6]1:[c:7]2:[#7;a:8]:[c:9]:[#7;a:10](-[c:11]):[c:12]:2:[c:13](=[O;D1;H0:14]):[nH;D2;+0:15]:[c:16]:1=[O;D1;H0:17]>>[#8:2]-[C:3](=[O;D1;H0:4])-[C:5]-[#7;a:6]1:[c:7]2:[#7;a:8]:[c:9]:[#7;a:10](-[c:11]):[c:12]:2:[c:13](=[O;D1;H0:14]):[n;H0;D3;+0:15](-[CH3;D1;+0:1]):[c:16...
77.9
[{"value": 77.9, "product": "C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2N(C(N(C(C2N1C1=C(C=CC=C1)C=C)=O)C)=O)CC(=O)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
13
HOUR
4-[3-Ethoxycarbonylmethyl-2,6-dioxo-7-(2-vinylphenyl)-2,3,6,7-tetrahydro-1H-purin-8-yl]piperazine-1-carboxylic acid tert-butyl ester (60 mg) was dissolved in N,N-dimethylformamide (2 ml), methyl iodide (17 μl) and potassium carbonate (17 mg) were added to the solution, and the mixture was stirred at room temperature fo...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ncc2[nH]cnc2n1
c1ncc2[nH]cnc2n1
c1ccccc1.C1C[NH]CC[NH]1.c1ncc2[nH]cnc2n1
HI
CN(C=O)C.C(C)(=O)OCC
null
13
C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)[nH]c(=O)n2CC(=O)OCC.CI>CN(C=O)C.C(C)(=O)OCC>C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(C)c(=O)n2CC(=O)OCC
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ff900d9875734a6a9c281ddf5fcf81de
C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(C)c(=O)n2CC(=O)OCC>>C=Cc1ccccc1-n1c(N2CCNCC2)nc2c1c(=O)n(C)c(=O)n2CC(=O)OCC
C(C)(C)(C)OC(=O)N1CCN(CC1)C1=NC=2N(C(N(C(C2N1C1=C(C=CC=C1)C=C)=O)C)=O)CC(=O)OCC.FC(C(=O)O)(F)F>>FC(C(=O)O)(F)F.C(C)OC(CN1C(N(C(C=2N(C(=NC12)N1CCNCC1)C1=C(C=CC=C1)C=C)=O)C)=O)=O
CC(C)(C)OC(=O)[N:14]1[CH2:13][CH2:12][N:11]([c:10]2[n:9](-[c:8]3[c:3]([CH:2]=[CH2:1])[cH:4][cH:5][cH:6][cH:7]3)[c:19]3[c:18]([n:17]2)[n:26]([CH2:27][C:28](=[O:29])[O:30][CH2:31][CH3:32])[c:24](=[O:25])[n:22]([CH3:23])[c:20]3=[O:21])[CH2:16][CH2:15]1>>[CH2:1]=[CH:2][c:3]1[cH:4][cH:5][cH:6][cH:7][c:8]1-[n:9]1[c:10]([N:11...
C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(C)c(=O)n2CC(=O)OCC
C=Cc1ccccc1-n1c(N2CCNCC2)nc2c1c(=O)n(C)c(=O)n2CC(=O)OCC
null
null
null
Reduction
Boc amine deprotection
2c25e19aee181a3c5131cfdfda27035fd54d4379a11d745dfb75d386bacfd500
a94b29c7264c852156fc1cdd4a0951a4fc26c06d0edc9e50c743825dbf79e3fd
O=c1[nH]c(=O)c2c(nc(N3CCNCC3)n2-c2ccccc2)[nH]1
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1]1-[C:2]-[C:3]-[#7:4]-[C:5]-[C:6]-1>>[#7:4]1-[C:3]-[C:2]-[NH;D2;+0:1]-[C:6]-[C:5]-1
null
[]
null
null
null
null
4-[3-Ethoxycarbonylmethyl-1-methyl-2,6-dioxo-7-(2-vinylphenyl)-2,3,6,7-tetrahydro-1H-purin-8-yl]piperazine-1-carboxylic acid tert-butyl ester (8 mg) was dissolved in trifluoroacetic acid and the solution was concentrated. The residue was purified by reversed phase high performance liquid chromatography to give 2.68 mg ...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Secondary amine
C1C[NH]CC[NH]1
C1C[NH]CCN1
c1ccccc1.C1C[NH]CCN1.c1ncc2[nH]cnc2n1
HO-
null
null
null
C=Cc1ccccc1-n1c(N2CCN(C(=O)OC(C)(C)C)CC2)nc2c1c(=O)n(C)c(=O)n2CC(=O)OCC>>C=Cc1ccccc1-n1c(N2CCNCC2)nc2c1c(=O)n(C)c(=O)n2CC(=O)OCC
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d5c834b6634d45bfba14c26c79f7b31d
Cc1ccc(O)cc1.Nc1ccccc1[N+](=O)[O-]>>Cc1ccc(O)c(N=Nc2ccccc2[N+](=O)[O-])c1
CCC(CC)COC(C1=CC=CC=C1)(C2=CC=CC=C2)C(=O)N(C)CC[NH+](C)C.[Cl-].N(=O)OS(O)(=O)=O.[N+](=O)([O-])C1=C(N)C=CC=C1.C1=CC(=CC=C1O)C.CCC(CC)COC(C1=CC=CC=C1)(C2=CC=CC=C2)C(=O)N(C)CC[NH+](C)C.[Cl-]>>[N+](=O)([O-])C1=C(C=CC=C1)N=NC1=C(C=CC(=C1)C)O
[CH3:1][c:2]1[cH:3][cH:4][c:5]([OH:6])[cH:7][cH:19]1.[NH2:9][c:10]1[cH:11][cH:12][cH:13][cH:14][c:15]1[N+:16](=[O:17])[O-:18]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([OH:6])[c:7]([N:8]=[N:9][c:10]2[cH:11][cH:12][cH:13][cH:14][c:15]2[N+:16](=[O:17])[O-:18])[cH:19]1
Cc1ccc(O)cc1.Nc1ccccc1[N+](=O)[O-]
Cc1ccc(O)c(N=Nc2ccccc2[N+](=O)[O-])c1
null
null
O.S(O)(O)(=O)=O
Functional Group Addition
OtherReaction
4dfa1e0075917e3f76a2c771d85af2eb7328e8c1dacc2fef053ab9d7871727bb
369e32a405523c63be3b198dc14b1fa8567bb17806d598f8dc85ecca177f9307
c1ccc(N=Nc2ccccc2)cc1
[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4].[O;D1;H1:5]-[c:6](:[c:7]):[cH;D2;+0:8]:[c:9]:[c:10]>>[O;D1;H1:5]-[c:6](:[c:7]):[c;H0;D3;+0:8](-[#7:11]=[N;H0;D2;+0:1]-[c:2](:[c:3]):[c:4]):[c:9]:[c:10]
null
[]
50
CELSIUS
15
MINUTE
A mixture of 2-nitroaniline (27.63 g, 0.2 mol), para-cresol (10.81 g, 0.10 mol), Hostapur® SAS93 (1.55), Triton X-100® [polyethylene(10) isooctylphenyl ether] (2.45 g) and water (100 mL) is heated to 50° C. The reaction mixture is rapidly stirred at this temperature for 15 minutes and then the rapidly stirred resultant...
10.6084/m9.figshare.5104873.v1
null
Primary amine
Diazene
c1ccccc1
c1ccccc1
c1ccccc1.c1ccccc1
Other
O.S(O)(O)(=O)=O
50
0.25
Cc1ccc(O)cc1.Nc1ccccc1[N+](=O)[O-]>O.S(O)(O)(=O)=O>Cc1ccc(O)c(N=Nc2ccccc2[N+](=O)[O-])c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-54712e92bae34a0a8db4cc695beda680
CC(C)(C)[Si](C)(C)Cl.CC(C)C(=O)Nc1nc2c(ncn2[C@H]2C[C@H](O)[C@@H](CO)O2)c(=O)[nH]1>>CC(C)C(=O)Nc1nc2c(ncn2[C@H]2C[C@H](O)[C@@H](CO[Si](C)(C)C(C)(C)C)O2)c(=O)[nH]1
C(C(C)C)(=O)NC=1NC(C=2N=CN([C@H]3C[C@H](O)[C@@H](CO)O3)C2N1)=O.N1C=NC=C1.[Si](C)(C)(C(C)(C)C)Cl>>C(C(C)C)(=O)NC=1NC(C=2N=CN([C@H]3C[C@H](O)[C@@H](CO[Si](C)(C)C(C)(C)C)O3)C2N1)=O
Cl[Si:21]([CH3:22])([CH3:23])[C:24]([CH3:25])([CH3:26])[CH3:27].[CH3:1][CH:2]([CH3:3])[C:4](=[O:5])[NH:6][c:7]1[n:8][c:9]2[c:10]([n:11][cH:12][n:13]2[C@H:14]2[CH2:15][C@H:16]([OH:17])[C@@H:18]([CH2:19][OH:20])[O:28]2)[c:29](=[O:30])[nH:31]1>>[CH3:1][CH:2]([CH3:3])[C:4](=[O:5])[NH:6][c:7]1[n:8][c:9]2[c:10]([n:11][cH:12]...
CC(C)(C)[Si](C)(C)Cl.CC(C)C(=O)Nc1nc2c(ncn2[C@H]2C[C@H](O)[C@@H](CO)O2)c(=O)[nH]1
CC(C)C(=O)Nc1nc2c(ncn2[C@H]2C[C@H](O)[C@@H](CO[Si](C)(C)C(C)(C)C)O2)c(=O)[nH]1
null
null
CN(C)C=O
Protection
Alcohol protection with silyl ethers
0085cd6629412592263fdf1537bdf8c19ef10dbeafe6f880807464d8107fa715
d2a170d01b2f3ec57d6fac058519475050ba5531f5d304635fb42e153d5bb9b5
O=c1[nH]cnc2c1ncn2[C@H]1CCCO1
Cl-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[C:4](-[C;D1;H3:5])(-[C;D1;H3:6])-[C;D1;H3:7].[#8:8]-[C:9]-[C:10]-[OH;D1;+0:11]>>[#8:8]-[C:9]-[C:10]-[O;H0;D2;+0:11]-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[C:4](-[C;D1;H3:5])(-[C;D1;H3:6])-[C;D1;H3:7]
74.7
[{"value": 74.0, "product": "C(C(C)C)(=O)NC=1NC(C=2N=CN([C@H]3C[C@H](O)[C@@H](CO[Si](C)(C)C(C)(C)C)O3)C2N1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 74.7, "product": "C(C(C)C)(=O)NC=1NC(C=2N=CN([C@H]3C[C@H](O)[C@@H](CO[Si](C)(C)C(C)(C)C)O3)C2N1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired...
null
null
8
HOUR
N2-isobutyryl-2′-deoxyguanosine (20.5 g) was dissolved in 200 ml of DMF. After 18.5 g of imidazole was dissolved in the resultant solution by addition, 21.4 g of tert-butyldimethylsilyl chloride was then added. DMF (100 ml) was further added and the solution was stirred at room temperature. After 8 hours, extraction us...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Silyl protective group
TMS ether protective group
null
null
c1ncc2[nH]cnc2n1.C1CCOC1
HCl
CN(C)C=O
null
8
CC(C)(C)[Si](C)(C)Cl.CC(C)C(=O)Nc1nc2c(ncn2[C@H]2C[C@H](O)[C@@H](CO)O2)c(=O)[nH]1>CN(C)C=O>CC(C)C(=O)Nc1nc2c(ncn2[C@H]2C[C@H](O)[C@@H](CO[Si](C)(C)C(C)(C)C)O2)c(=O)[nH]1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c98c3a80fa4e45bcbe3bfa72698996ee
CC(C)C(=O)Nc1nc2c(ncn2[C@H]2C[C@H](O)[C@@H](CO[Si](C)(C)C(C)(C)C)O2)c(=O)[nH]1.COc1ccc(C(Cl)(c2ccccc2)c2ccc(OC)cc2)cc1>>COc1ccc(C(O[C@H]2C[C@H](n3cnc4c(=O)[nH]c(NC(=O)C(C)C)nc43)O[C@@H]2CO[Si](C)(C)C(C)(C)C)(c2ccccc2)c2ccc(OC)cc2)cc1
C(O)([O-])=O.[Na+].COC1=CC=C(C(C2=CC=C(C=C2)OC)(C2=CC=CC=C2)Cl)C=C1.C(C(C)C)(=O)NC=1NC(C=2N=CN([C@H]3C[C@H](O)[C@@H](CO[Si](C)(C)C(C)(C)C)O3)C2N1)=O>>C(C(C)C)(=O)NC=1NC(C=2N=CN([C@H]3C[C@H](OC(C4=CC=C(C=C4)OC)(C4=CC=C(C=C4)OC)C4=CC=CC=C4)[C@@H](CO[Si](C)(C)C(C)(C)C)O3)C2N1)=O
[OH:8][C@H:9]1[CH2:10][C@H:11]([n:12]2[cH:13][n:14][c:15]3[c:16](=[O:17])[nH:18][c:19]([NH:20][C:21](=[O:22])[CH:23]([CH3:24])[CH3:25])[n:26][c:27]23)[O:28][C@@H:29]1[CH2:30][O:31][Si:32]([CH3:33])([CH3:34])[C:35]([CH3:36])([CH3:37])[CH3:38].Cl[C:7]([c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:54][cH:53]1)([c:39]1[cH:40][c...
CC(C)C(=O)Nc1nc2c(ncn2[C@H]2C[C@H](O)[C@@H](CO[Si](C)(C)C(C)(C)C)O2)c(=O)[nH]1.COc1ccc(C(Cl)(c2ccccc2)c2ccc(OC)cc2)cc1
COc1ccc(C(O[C@H]2C[C@H](n3cnc4c(=O)[nH]c(NC(=O)C(C)C)nc43)O[C@@H]2CO[Si](C)(C)C(C)(C)C)(c2ccccc2)c2ccc(OC)cc2)cc1
null
null
N1=CC=CC=C1
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
5ab68839e2c0c36dcda93f3c0a707140e3d24e3e006f5c14702a7b8884a9a81e
26c50c761bd192b9bbaacc80ceb1f72503dc7c2f688b52834534ac0a03b55cce
O=c1[nH]cnc2c1ncn2[C@H]1C[C@H](OC(c2ccccc2)(c2ccccc2)c2ccccc2)CO1
Cl-[C;H0;D4;+0:1](-[c:2](:[c:3]):[c:4])(-[c:5](:[c:6]):[c:7])-[c:8](:[c:9]):[c:10].[#8:11]-[C:12]-[C:13](-[OH;D1;+0:14])-[C:15]>>[#8:11]-[C:12]-[C:13](-[O;H0;D2;+0:14]-[C;H0;D4;+0:1](-[c:2](:[c:3]):[c:4])(-[c:5](:[c:6]):[c:7])-[c:8](:[c:9]):[c:10])-[C:15]
698.5
[{"value": 78.0, "product": "C(C(C)C)(=O)NC=1NC(C=2N=CN([C@H]3C[C@H](OC(C4=CC=C(C=C4)OC)(C4=CC=C(C=C4)OC)C4=CC=CC=C4)[C@@H](CO[Si](C)(C)C(C)(C)C)O3)C2N1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 698.5, "product": "C(C(C)C)(=O)NC=1NC(C=2N=CN([C@H]3C[C@H](OC(C4=CC=C(C=C4)OC)(C4=CC=C(C=C4)OC)C4=CC=CC...
40
CELSIUS
null
null
N2-isobutyryl-5′-O-(tert-butyldimethylsilyl)-2′-deoxyguanosine (19.8 g) was dissolved in 100 ml of anhydrous pyridine. 4,4′-dimethoxytrityl chloride (1.66 g) was added to the resultant solution and 140 ml of anhydrous pyridine was further added, follow by stirring at 40° C. After the reaction completed, the reaction mi...
10.6084/m9.figshare.5104873.v1
null
Tertiary halide.Secondary alcohol
Ether
null
null
c1ccccc1.C1CCOC1.c1ncc2nc[nH]c2n1.c1ccccc1.c1ccccc1
HCl
N1=CC=CC=C1
40
null
CC(C)C(=O)Nc1nc2c(ncn2[C@H]2C[C@H](O)[C@@H](CO[Si](C)(C)C(C)(C)C)O2)c(=O)[nH]1.COc1ccc(C(Cl)(c2ccccc2)c2ccc(OC)cc2)cc1>N1=CC=CC=C1>COc1ccc(C(O[C@H]2C[C@H](n3cnc4c(=O)[nH]c(NC(=O)C(C)C)nc43)O[C@@H]2CO[Si](C)(C)C(C)(C)C)(c2ccccc2)c2ccc(OC)cc2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f5a4db9a237d4cf9997ec58c3924f4fb
CC(C)(C)[Si](C)(C)Cl.O=C(Nc1ncnc2c1ncn2[C@H]1C[C@H](O)[C@@H](CO)O1)c1ccccc1>>CC(C)(C)[Si](C)(C)OC[C@H]1O[C@@H](n2cnc3c(NC(=O)c4ccccc4)ncnc32)C[C@@H]1O
[Si](C)(C)(C(C)(C)C)Cl.N1C=NC=C1.C(C1=CC=CC=C1)(=O)NC=1C=2N=CN([C@H]3C[C@H](O)[C@@H](CO)O3)C2N=CN1>>C(C1=CC=CC=C1)(=O)NC=1C=2N=CN([C@H]3C[C@H](O)[C@@H](CO[Si](C)(C)C(C)(C)C)O3)C2N=CN1
Cl[Si:5]([C:2]([CH3:1])([CH3:3])[CH3:4])([CH3:6])[CH3:7].[OH:8][CH2:9][C@H:10]1[O:11][C@@H:12]([n:13]2[cH:14][n:15][c:16]3[c:17]([NH:18][C:19](=[O:20])[c:21]4[cH:22][cH:23][cH:24][cH:25][cH:26]4)[n:27][cH:28][n:29][c:30]23)[CH2:31][C@@H:32]1[OH:33]>>[CH3:1][C:2]([CH3:3])([CH3:4])[Si:5]([CH3:6])([CH3:7])[O:8][CH2:9][C@H...
CC(C)(C)[Si](C)(C)Cl.O=C(Nc1ncnc2c1ncn2[C@H]1C[C@H](O)[C@@H](CO)O1)c1ccccc1
CC(C)(C)[Si](C)(C)OC[C@H]1O[C@@H](n2cnc3c(NC(=O)c4ccccc4)ncnc32)C[C@@H]1O
null
null
CN(C)C=O
Protection
Alcohol protection with silyl ethers
0085cd6629412592263fdf1537bdf8c19ef10dbeafe6f880807464d8107fa715
d2a170d01b2f3ec57d6fac058519475050ba5531f5d304635fb42e153d5bb9b5
O=C(Nc1ncnc2c1ncn2[C@H]1CCCO1)c1ccccc1
Cl-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[C:4](-[C;D1;H3:5])(-[C;D1;H3:6])-[C;D1;H3:7].[#8:8]-[C:9]-[C:10]-[OH;D1;+0:11]>>[#8:8]-[C:9]-[C:10]-[O;H0;D2;+0:11]-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[C:4](-[C;D1;H3:5])(-[C;D1;H3:6])-[C;D1;H3:7]
61
[{"value": 61.0, "product": "C(C1=CC=CC=C1)(=O)NC=1C=2N=CN([C@H]3C[C@H](O)[C@@H](CO[Si](C)(C)C(C)(C)C)O3)C2N=CN1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 58.2, "product": "C(C1=CC=CC=C1)(=O)NC=1C=2N=CN([C@H]3C[C@H](O)[C@@H](CO[Si](C)(C)C(C)(C)C)O3)C2N=CN1", "details": "CALCULATEDPERCENTYIELD", "is_d...
null
null
8
HOUR
N6-benzoyl-2′-deoxyadenosine (20.95 g) was dissolved in 200 ml of DMF. Imidazole (15.7 g) was dissolved to the resultant solution by addition. Then, 20.8 g of tert-butyldimethylsilyl chloride was added. DMF (100 ml) was further added and the solution was stirred at room temperature. After 8 hours, extraction using chlo...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Silyl protective group
TMS ether protective group
null
null
C1CCOC1.c1ccccc1.c1ncnc2[nH]cnc12
HCl
CN(C)C=O
null
8
CC(C)(C)[Si](C)(C)Cl.O=C(Nc1ncnc2c1ncn2[C@H]1C[C@H](O)[C@@H](CO)O1)c1ccccc1>CN(C)C=O>CC(C)(C)[Si](C)(C)OC[C@H]1O[C@@H](n2cnc3c(NC(=O)c4ccccc4)ncnc32)C[C@@H]1O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-18c7ff5220a5423189fd868f41a6727a
CC(C)(C)[Si](C)(C)OC[C@H]1O[C@@H](n2cnc3c(NC(=O)c4ccccc4)ncnc32)C[C@@H]1O.COc1ccc(C(Cl)(c2ccccc2)c2ccc(OC)cc2)cc1>>COc1ccc(C(O[C@H]2C[C@H](n3cnc4c(NC(=O)c5ccccc5)ncnc43)O[C@@H]2CO[Si](C)(C)C(C)(C)C)(c2ccccc2)c2ccc(OC)cc2)cc1
C(C1=CC=CC=C1)(=O)NC=1C=2N=CN([C@H]3C[C@H](O)[C@@H](CO[Si](C)(C)C(C)(C)C)O3)C2N=CN1.COC1=CC=C(C(C2=CC=C(C=C2)OC)(C2=CC=CC=C2)Cl)C=C1.C(O)([O-])=O.[Na+]>>C(C1=CC=CC=C1)(=O)NC=1C=2N=CN([C@H]3C[C@H](OC(C4=CC=C(C=C4)OC)(C4=CC=C(C=C4)OC)C4=CC=CC=C4)[C@@H](CO[Si](C)(C)C(C)(C)C)O3)C2N=CN1
[OH:8][C@H:9]1[CH2:10][C@H:11]([n:12]2[cH:13][n:14][c:15]3[c:16]([NH:17][C:18](=[O:19])[c:20]4[cH:21][cH:22][cH:23][cH:24][cH:25]4)[n:26][cH:27][n:28][c:29]23)[O:30][C@@H:31]1[CH2:32][O:33][Si:34]([CH3:35])([CH3:36])[C:37]([CH3:38])([CH3:39])[CH3:40].Cl[C:7]([c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:56][cH:55]1)([c:41]1...
CC(C)(C)[Si](C)(C)OC[C@H]1O[C@@H](n2cnc3c(NC(=O)c4ccccc4)ncnc32)C[C@@H]1O.COc1ccc(C(Cl)(c2ccccc2)c2ccc(OC)cc2)cc1
COc1ccc(C(O[C@H]2C[C@H](n3cnc4c(NC(=O)c5ccccc5)ncnc43)O[C@@H]2CO[Si](C)(C)C(C)(C)C)(c2ccccc2)c2ccc(OC)cc2)cc1
null
null
N1=CC=CC=C1
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
5ab68839e2c0c36dcda93f3c0a707140e3d24e3e006f5c14702a7b8884a9a81e
26c50c761bd192b9bbaacc80ceb1f72503dc7c2f688b52834534ac0a03b55cce
O=C(Nc1ncnc2c1ncn2[C@H]1C[C@H](OC(c2ccccc2)(c2ccccc2)c2ccccc2)CO1)c1ccccc1
Cl-[C;H0;D4;+0:1](-[c:2](:[c:3]):[c:4])(-[c:5](:[c:6]):[c:7])-[c:8](:[c:9]):[c:10].[#8:11]-[C:12]-[C:13](-[OH;D1;+0:14])-[C:15]>>[#8:11]-[C:12]-[C:13](-[O;H0;D2;+0:14]-[C;H0;D4;+0:1](-[c:2](:[c:3]):[c:4])(-[c:5](:[c:6]):[c:7])-[c:8](:[c:9]):[c:10])-[C:15]
63.1
[{"value": 63.0, "product": "C(C1=CC=CC=C1)(=O)NC=1C=2N=CN([C@H]3C[C@H](OC(C4=CC=C(C=C4)OC)(C4=CC=C(C=C4)OC)C4=CC=CC=C4)[C@@H](CO[Si](C)(C)C(C)(C)C)O3)C2N=CN1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 63.1, "product": "C(C1=CC=CC=C1)(=O)NC=1C=2N=CN([C@H]3C[C@H](OC(C4=CC=C(C=C4)OC)(C4=CC=C(C=C4)OC)C4=...
45
CELSIUS
null
null
N6-benzoyl-5′-O-(tert-butyldimethylsilyl)-2′-deoxyadenosine (16.1 g) was dissolved in 100 ml of anhydrous pyridine. 4,4′-dimethoxytrityl chloride (12.8 g) and anhydrous pyridine (140 ml) were further added, follow by stirring at 45° C. After the reaction completed, the reaction mixture was neutralized by sodium hydroge...
10.6084/m9.figshare.5104873.v1
null
Tertiary halide.Secondary alcohol
Ether
null
null
c1ccccc1.C1CCOC1.c1ccccc1.c1ncnc2[nH]cnc12.c1ccccc1.c1ccccc1
HCl
N1=CC=CC=C1
45
null
CC(C)(C)[Si](C)(C)OC[C@H]1O[C@@H](n2cnc3c(NC(=O)c4ccccc4)ncnc32)C[C@@H]1O.COc1ccc(C(Cl)(c2ccccc2)c2ccc(OC)cc2)cc1>N1=CC=CC=C1>COc1ccc(C(O[C@H]2C[C@H](n3cnc4c(NC(=O)c5ccccc5)ncnc43)O[C@@H]2CO[Si](C)(C)C(C)(C)C)(c2ccccc2)c2ccc(OC)cc2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-02a4ff65175446a9b2d8b8655bce1c71
COc1ccc(C(O[C@H]2C[C@H](n3cnc4c(NC(=O)c5ccccc5)ncnc43)O[C@@H]2CO[Si](C)(C)C(C)(C)C)(c2ccccc2)c2ccc(OC)cc2)cc1>>COc1ccc(C(O[C@H]2C[C@H](n3cnc4c(NC(=O)c5ccccc5)ncnc43)O[C@@H]2CO)(c2ccccc2)c2ccc(OC)cc2)cc1
[F-].C(CCC)[N+](CCCC)(CCCC)CCCC.C(C1=CC=CC=C1)(=O)NC=1C=2N=CN([C@H]3C[C@H](OC(C4=CC=C(C=C4)OC)(C4=CC=C(C=C4)OC)C4=CC=CC=C4)[C@@H](CO[Si](C)(C)C(C)(C)C)O3)C2N=CN1>>C(C1=CC=CC=C1)(=O)NC=1C=2N=CN([C@H]3C[C@H](OC(C4=CC=C(C=C4)OC)(C4=CC=C(C=C4)OC)C4=CC=CC=C4)[C@@H](CO)O3)C2N=CN1
CC(C)(C)[Si](C)(C)[O:33][CH2:32][C@@H:31]1[C@@H:9]([O:8][C:7]([c:6]2[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:49][cH:48]2)([c:34]2[cH:35][cH:36][cH:37][cH:38][cH:39]2)[c:40]2[cH:41][cH:42][c:43]([O:44][CH3:45])[cH:46][cH:47]2)[CH2:10][C@H:11]([n:12]2[cH:13][n:14][c:15]3[c:16]([NH:17][C:18](=[O:19])[c:20]4[cH:21][cH:22][cH:23]...
COc1ccc(C(O[C@H]2C[C@H](n3cnc4c(NC(=O)c5ccccc5)ncnc43)O[C@@H]2CO[Si](C)(C)C(C)(C)C)(c2ccccc2)c2ccc(OC)cc2)cc1
COc1ccc(C(O[C@H]2C[C@H](n3cnc4c(NC(=O)c5ccccc5)ncnc43)O[C@@H]2CO)(c2ccccc2)c2ccc(OC)cc2)cc1
null
null
C1CCOC1
Deprotection
Alcohol deprotection from silyl ethers
6ff8c9c41093ab5237b871dd4689ba6431022d615e227d3774901a983c846e4b
84d9f5b4e7757c58e584c26c7d52c9a3f594fbcb0c0d22f34765a93a932fcd5b
O=C(Nc1ncnc2c1ncn2[C@H]1C[C@H](OC(c2ccccc2)(c2ccccc2)c2ccccc2)CO1)c1ccccc1
C-C(-C)(-C)-[Si](-C)(-C)-[O;H0;D2;+0:1]-[C:2]-[C:3]-[#8:4]>>[#8:4]-[C:3]-[C:2]-[OH;D1;+0:1]
100
[{"value": 98.0, "product": "C(C1=CC=CC=C1)(=O)NC=1C=2N=CN([C@H]3C[C@H](OC(C4=CC=C(C=C4)OC)(C4=CC=C(C=C4)OC)C4=CC=CC=C4)[C@@H](CO)O3)C2N=CN1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 100.0, "product": "C(C1=CC=CC=C1)(=O)NC=1C=2N=CN([C@H]3C[C@H](OC(C4=CC=C(C=C4)OC)(C4=CC=C(C=C4)OC)C4=CC=CC=C4)[C@@H](C...
null
null
8
HOUR
N6-benzoyl-5′-O-(tert-butyldimethylsilyl)-3′-O-(4,4′-dimethoxytrityl)-2′-deoxyadenosine (16.2 g) was dissolved in 200 ml of dry THF. A THF solution (31 ml) of tetrabutylammonium fluoride was added to the resultant solution and 100 ml of dry THF was further added, followed by stirring at room temperature. After 8 hours,...
10.6084/m9.figshare.5104873.v1
null
TMS ether protective group
Primary alcohol
null
null
c1ccccc1.C1CCOC1.c1ccccc1.c1ncnc2[nH]cnc12.c1ccccc1.c1ccccc1
Other
C1CCOC1
null
8
COc1ccc(C(O[C@H]2C[C@H](n3cnc4c(NC(=O)c5ccccc5)ncnc43)O[C@@H]2CO[Si](C)(C)C(C)(C)C)(c2ccccc2)c2ccc(OC)cc2)cc1>C1CCOC1>COc1ccc(C(O[C@H]2C[C@H](n3cnc4c(NC(=O)c5ccccc5)ncnc43)O[C@@H]2CO)(c2ccccc2)c2ccc(OC)cc2)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-417447cdb51a438bb0b0932df74ca360
CC(=O)OCCBr.CCn1c(=O)[nH]c2ncn(Cc3ccc(OC)cc3)c2c1=O>>CCn1c(=O)c2c(ncn2Cc2ccc(OC)cc2)n(CCOC(C)=O)c1=O
C(C)N1C(NC=2N=CN(C2C1=O)CC1=CC=C(C=C1)OC)=O.C([O-])([O-])=O.[K+].[K+].C(C)(=O)OCCBr>>C(C)(=O)OCCN1C(N(C(C=2N(C=NC12)CC1=CC=C(C=C1)OC)=O)CC)=O
Br[CH2:21][CH2:22][O:23][C:24]([CH3:25])=[O:26].[CH3:1][CH2:2][n:3]1[c:4](=[O:5])[c:6]2[c:7]([n:8][cH:9][n:10]2[CH2:11][c:12]2[cH:13][cH:14][c:15]([O:16][CH3:17])[cH:18][cH:19]2)[nH:20][c:27]1=[O:28]>>[CH3:1][CH2:2][n:3]1[c:4](=[O:5])[c:6]2[c:7]([n:8][cH:9][n:10]2[CH2:11][c:12]2[cH:13][cH:14][c:15]([O:16][CH3:17])[cH:1...
CC(=O)OCCBr.CCn1c(=O)[nH]c2ncn(Cc3ccc(OC)cc3)c2c1=O
CCn1c(=O)c2c(ncn2Cc2ccc(OC)cc2)n(CCOC(C)=O)c1=O
null
S(=O)(=O)(O)[O-].C(CCC)[N+](CCCC)(CCCC)CCCC
C(C)#N
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
453c185c7ca08f316f04eb7765c2f018ec3b56836368f5fa1ad0e7a49cf724d8
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
O=c1[nH]c(=O)c2c(ncn2Cc2ccccc2)[nH]1
Br-[CH2;D2;+0:1]-[C:2]-[#8:3]-[C:4](-[C;D1;H3:5])=[O;D1;H0:6].[C:7]-[#7;a:8]1:[c:9]:[#7;a:10]:[c:11]2:[nH;D2;+0:12]:[c:13](=[O;D1;H0:14]):[#7;a:15](-[C:16]):[c:17]:[c:18]:1:2>>[C:7]-[#7;a:8]1:[c:9]:[#7;a:10]:[c:11]2:[c:18]:1:[c:17]:[#7;a:15](-[C:16]):[c:13](=[O;D1;H0:14]):[n;H0;D3;+0:12]:2-[CH2;D2;+0:1]-[C:2]-[#8:3]-[C...
75
[{"value": 75.0, "product": "C(C)(=O)OCCN1C(N(C(C=2N(C=NC12)CC1=CC=C(C=C1)OC)=O)CC)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
7
HOUR
Acetonitrile was added to a mixture of Compound 5A (about 1.0 mole), anhydrous potassium carbonate (about 1.5 moles) and tetrabutylammonium hydrogen sulfate (about 0.05 mole). 2-bromoethyl acetate (about 1.5 moles) was added in three separate portions (0.72 mole in the beginning, another 0.45 mole after about 2 hours o...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ncc2nc[nH]c2n1
c1ncc2nc[nH]c2n1
c1ncc2nc[nH]c2n1.c1ccccc1
HBr
S(=O)(=O)(O)[O-].C(CCC)[N+](CCCC)(CCCC)CCCC.C(C)#N
null
7
CC(=O)OCCBr.CCn1c(=O)[nH]c2ncn(Cc3ccc(OC)cc3)c2c1=O>S(=O)(=O)(O)[O-].C(CCC)[N+](CCCC)(CCCC)CCCC.C(C)#N>CCn1c(=O)c2c(ncn2Cc2ccc(OC)cc2)n(CCOC(C)=O)c1=O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-6e4fce7737e24aebbe5a46ccc285cb6d
CCn1c(=O)c2c(nc(Br)n2Cc2ccc(OC)c(Br)c2)n(CCOC(C)=O)c1=O.N[C@@H]1CCC[C@H]1O>>CCn1c(=O)c2c(nc(NC3CCCC3O)n2Cc2ccc(OC)c(Br)c2)n(CCO)c1=O
[OH-].C(CCC)[N+](CCCC)(CCCC)CCCC.BrC1=NC=2N(C(N(C(C2N1CC1=CC(=C(C=C1)OC)Br)=O)CC)=O)CCOC(C)=O.Cl.N[C@H]1[C@@H](CCC1)O.C([O-])(O)=O.[Na+].Cl.N[C@H]1[C@@H](CCC1)O>>CCN1C(=O)C2=C(N=C(N2CC3=CC(=C(C=C3)OC)Br)NC4CCCC4O)N(C1=O)CCO
CC(=O)[O:31][CH2:30][CH2:29][n:28]1[c:7]2[c:6]([c:4](=[O:5])[n:3]([CH2:2][CH3:1])[c:32]1=[O:33])[n:17]([CH2:18][c:19]1[cH:20][cH:21][c:22]([O:23][CH3:24])[c:25]([Br:26])[cH:27]1)[c:9](Br)[n:8]2.[NH2:10][C@@H:11]1[CH2:12][CH2:13][CH2:14][C@H:15]1[OH:16]>>[CH3:1][CH2:2][n:3]1[c:4](=[O:5])[c:6]2[c:7]([n:8][c:9]([NH:10][CH...
CCn1c(=O)c2c(nc(Br)n2Cc2ccc(OC)c(Br)c2)n(CCOC(C)=O)c1=O.N[C@@H]1CCC[C@H]1O
CCn1c(=O)c2c(nc(NC3CCCC3O)n2Cc2ccc(OC)c(Br)c2)n(CCO)c1=O
null
null
O.CO.CN(C(C)=O)C
Heteroatom Alkylation and Arylation
OtherReaction
3f5a6a497ea9d80a6bc5e13a61301a854ae9c711f0d3b07c7e15d9b1d01480a9
03164802232677317a7efd0e24d53056dbf9714f8e35a1ee2da95661003b43d6
O=c1[nH]c(=O)c2c(nc(NC3CCCC3)n2Cc2ccccc2)[nH]1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]2:[#7;a:4](-[C:5]-[C:6]-[O;H0;D2;+0:7]-C(-C)=O):[c:8]:[#7;a:9]:[c:10]:[c:11]:2:[#7;a:12]:1-[C:13].[NH2;D1;+0:14]-[C@@H;D3;+0:15]1-[C:16]-[C:17]-[C:18]-[C@H;D3;+0:19]-1-[O;D1;H1:20]>>[C:13]-[#7;a:12]1:[c:11]2:[c:10]:[#7;a:9]:[c:8]:[#7;a:4](-[C:5]-[C:6]-[OH;D1;+0:7]):[c:3]:2:[#7;a:2]:[c;H...
85
[{"value": 85.0, "product": "CCN1C(=O)C2=C(N=C(N2CC3=CC(=C(C=C3)OC)Br)NC4CCCC4O)N(C1=O)CCO", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
Compound 7A (about 1 mole) was combined with (R,R)-2-amino-1-cyclopentanol hydrochloride (Compound 8A, about 1.2 moles) and sodium bicarbonate (about 3 moles). To this reaction mixture was added N,N-dimethylacetamide (“DMA”), and the reaction mixture was agitated at about 135–140° C. for about 15–17 hours until complet...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Primary amine
Primary alcohol.Secondary amine
c1ncc2[nH]cnc2n1
c1ncc2nc[nH]c2n1
c1ncc2nc[nH]c2n1.C1CCCC1.c1ccccc1
HBr
O.CO.CN(C(C)=O)C
null
null
CCn1c(=O)c2c(nc(Br)n2Cc2ccc(OC)c(Br)c2)n(CCOC(C)=O)c1=O.N[C@@H]1CCC[C@H]1O>O.CO.CN(C(C)=O)C>CCn1c(=O)c2c(nc(NC3CCCC3O)n2Cc2ccc(OC)c(Br)c2)n(CCO)c1=O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-52b64d49f97e460aaf28e0d6614f1d05
COC(=O)Cl.CON1C(=O)[C@H](N)Cc2ccccc21>>COC(=O)N[C@@H]1Cc2ccccc2N(OC)C1=O
ClC(=O)OC.CON1C([C@@H](CC2=CC=CC=C12)N)=O.C([O-])(O)=O.[Na+]>>CON1C([C@@H](CC2=CC=CC=C12)NC(OC)=O)=O
Cl[C:3]([O:2][CH3:1])=[O:4].[NH2:5][C@@H:6]1[CH2:7][c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]2[N:14]([O:15][CH3:16])[C:17]1=[O:18]>>[CH3:1][O:2][C:3](=[O:4])[NH:5][C@@H:6]1[CH2:7][c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]2[N:14]([O:15][CH3:16])[C:17]1=[O:18]
COC(=O)Cl.CON1C(=O)[C@H](N)Cc2ccccc21
COC(=O)N[C@@H]1Cc2ccccc2N(OC)C1=O
null
null
O.C(Cl)(Cl)Cl.CCCCC
Protection
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
038720aa61a7efa0f2a9ee6f2e0adf63a9ffdc2be4697c11a6215baef34f97b2
205f353513ce9506ab61831799da8fb73ec2ef5cfa927664496d3ce72c438860
O=C1CCc2ccccc2N1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C;D1;H3:4].[#8:5]-[#7:6](-[c:7])-[C:8](=[O;D1;H0:9])-[C:10](-[NH2;D1;+0:11])-[C:12]>>[#8:5]-[#7:6](-[c:7])-[C:8](=[O;D1;H0:9])-[C:10](-[NH;D2;+0:11]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C;D1;H3:4])-[C:12]
99
[{"value": 99.0, "product": "CON1C([C@@H](CC2=CC=CC=C12)NC(OC)=O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 98.6, "product": "CON1C([C@@H](CC2=CC=CC=C12)NC(OC)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
A solution of methyl chloroformate (42.8 g, 0.453 mol) in chloroform (50 ml) was added to a mixture of (R)-1,2,3,4-tetrahydro-1-methoxy-2-oxo-3-quinolinamine 1 (M. Kawase, T. Kitamura, Y. Kilugawa, J. Org. Chem., 54, 1989 3394–3403)(0.15 mol) and sodium bicarbonate (50.4 g, 0.600 mol) in chloroform (250 ml) and water (...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Ether.Primary amine
Carbamic ester
null
null
c1ccc2c(c1)CCC[NH]2
HCl
O.C(Cl)(Cl)Cl.CCCCC
null
8
COC(=O)Cl.CON1C(=O)[C@H](N)Cc2ccccc21>O.C(Cl)(Cl)Cl.CCCCC>COC(=O)N[C@@H]1Cc2ccccc2N(OC)C1=O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d343a18f0d5d4b3e83df4a271cf4b5d1
CCCI.CCCN[C@@H]1Cc2cccc3c2n(c(=O)n3OC)C1>>CCCN(CCC)[C@@H]1Cc2cccc3c2n(c(=O)n3OC)C1
ICCC.C(CC)N[C@H]1CN2C3=C(C=CC=C3C1)N(C2=O)OC.ICCC.C([O-])([O-])=O.[K+].[K+]>>C(CC)N([C@H]1CN2C3=C(C=CC=C3C1)N(C2=O)OC)CCC
I[CH2:5][CH2:6][CH3:7].[CH3:1][CH2:2][CH2:3][NH:4][C@@H:8]1[CH2:9][c:10]2[cH:11][cH:12][cH:13][c:14]3[c:15]2[n:16]([c:17](=[O:18])[n:19]3[O:20][CH3:21])[CH2:22]1>>[CH3:1][CH2:2][CH2:3][N:4]([CH2:5][CH2:6][CH3:7])[C@@H:8]1[CH2:9][c:10]2[cH:11][cH:12][cH:13][c:14]3[c:15]2[n:16]([c:17](=[O:18])[n:19]3[O:20][CH3:21])[CH2:2...
CCCI.CCCN[C@@H]1Cc2cccc3c2n(c(=O)n3OC)C1
CCCN(CCC)[C@@H]1Cc2cccc3c2n(c(=O)n3OC)C1
null
null
C(C)#N
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
6d58cac08ccced0a33ed16fbca180bc12aa011288d6476106d98a7b2cbc3d709
523d37155b42c8dc851abeddadebb241cdd90bdf649ba750c35e13c8c752d7b0
O=c1[nH]c2cccc3c2n1CCC3
I-[CH2;D2;+0:1]-[C:2]-[C;D1;H3:3].[#7;a:4]-[C:5]-[C:6](-[NH;D2;+0:7]-[C:8]-[C:9])-[C:10]>>[#7;a:4]-[C:5]-[C:6](-[N;H0;D3;+0:7](-[C:8]-[C:9])-[CH2;D2;+0:1]-[C:2]-[C;D1;H3:3])-[C:10]
90
[{"value": 90.0, "product": "C(CC)N([C@H]1CN2C3=C(C=CC=C3C1)N(C2=O)OC)CCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 80.5, "product": "C(CC)N([C@H]1CN2C3=C(C=CC=C3C1)N(C2=O)OC)CCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Following the procedure of Example 3, a mixture of (R)-5-Propylamino-1-methoxy-5,6-dihydro-4H-imidazo[4,5,1-ij]quinolin-2(1H)-one (8b, 0.93 g, 3.56 mmol), 1-iodopropane (3.05 g, 17.9 mmol), and potassium carbonate (1.97 g, 14.3 mmol) in acetonitrile (25 ml) was heated at reflux under nitrogen for 17 hours. 1-Iodopropan...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amine
Tertiary amine
null
null
c1cc2c3c(c1)ncn3CCC2
HI
C(C)#N
null
null
CCCI.CCCN[C@@H]1Cc2cccc3c2n(c(=O)n3OC)C1>C(C)#N>CCCN(CCC)[C@@H]1Cc2cccc3c2n(c(=O)n3OC)C1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-26e379d5dcb345a5aaef6391ab1e77f6
COC(=O)Cl.N[C@H](Cc1ccccc1)C(=O)O>>COC(=O)N[C@H](Cc1ccccc1)C(=O)O
[OH-].[Na+].Cl.ClC(=O)OC.N[C@H](CC1=CC=CC=C1)C(=O)O.[OH-].[Na+]>>COC(=O)N[C@@H](C(=O)O)CC1=CC=CC=C1
Cl[C:3]([O:2][CH3:1])=[O:4].[NH2:5][C@H:6]([CH2:7][c:8]1[cH:9][cH:10][cH:11][cH:12][cH:13]1)[C:14](=[O:15])[OH:16]>>[CH3:1][O:2][C:3](=[O:4])[NH:5][C@H:6]([CH2:7][c:8]1[cH:9][cH:10][cH:11][cH:12][cH:13]1)[C:14](=[O:15])[OH:16]
COC(=O)Cl.N[C@H](Cc1ccccc1)C(=O)O
COC(=O)N[C@H](Cc1ccccc1)C(=O)O
null
null
O1CCCC1.O
Protection
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
038720aa61a7efa0f2a9ee6f2e0adf63a9ffdc2be4697c11a6215baef34f97b2
205f353513ce9506ab61831799da8fb73ec2ef5cfa927664496d3ce72c438860
c1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C;D1;H3:4].[C:5]-[C:6](-[NH2;D1;+0:7])-[C:8](=[O;D1;H0:9])-[O;D1;H1:10]>>[C:5]-[C:6](-[NH;D2;+0:7]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C;D1;H3:4])-[C:8](=[O;D1;H0:9])-[O;D1;H1:10]
113.9
[{"value": 113.9, "product": "COC(=O)N[C@@H](C(=O)O)CC1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
A solution of D-phenylalanine (25.00 g, 0.151 mol) and sodium hydroxide (6.05 g, 0.151 mol) in water (170 ml) and tetrahydrofuran (225 ml) was cooled to −15° C., and a solution of methyl chloroformate (18.6 g, 0.197 mol) in tetrahydrofuran (50 ml) was added dropwise. When the addition was ˜half complete, a solution of ...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Ether.Primary amine
Carbamic ester
null
null
c1ccccc1
HCl
O1CCCC1.O
null
2
COC(=O)Cl.N[C@H](Cc1ccccc1)C(=O)O>O1CCCC1.O>COC(=O)N[C@H](Cc1ccccc1)C(=O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-9fab0b95071347f8b60fa53a156419c7
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
CC(=O)CC
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
54
[{"value": 54.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
Clopidogrel base (5.01 g, leq.) was dissolved in methylethyl ketone (MEK) (39.5 mL). Eighty percent aqueous sulfuric acid (0.74 mL, 0.66 eq.) was added to the solution at 20° C. The reaction mixture was heated to reflux temperature for 2 hours. Then, the solution was cooled to room temperature and half of the amount of...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
CC(=O)CC
null
null
O=S(=O)(O)O>CC(=O)CC>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-6a8a7e4d77f14818b71be6d65c5464e0
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
CC(=O)CC
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
82
[{"value": 82.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
67
HOUR
Clopidogrel base (4.27 g, 1 eq.) was dissolved in methylethyl ketone (MEK) (33.7 ml). Eighty percent aqueous sulfuric acid (1.03 ml, 1.1 eq.) was added to the solution at 20° C. The reaction mixture was heated to reflux temperature for 2 hours. Then, the solution was cooled to room temperature and stirred at this tempe...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
CC(=O)CC
null
67
O=S(=O)(O)O>CC(=O)CC>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-30d8debe6dd34c569a3ba14a104ccb1b
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
ClCCl
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
30
[{"value": 30.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
Clopidogrel base (3.73 g, leq.) was dissolved in dichloromethane (29.4 mL). Eighty percent aqueous sulfuric acid (0.55 ml, 0.66 eq.) was added to the solution at 20° C. The reaction mixture was heated to reflux temperature for 2 hours during which a precipitate was formed. Then, the solution was cooled to room temperat...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
ClCCl
null
null
O=S(=O)(O)O>ClCCl>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-7401e0220750462db219600f520c35aa
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
ClCCl
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
48
[{"value": 48.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
16
HOUR
Clopidogrel base (4.37 g, 1 eq.) was dissolved in dichloromethane (34.5 mL). Eighty percent aqueous sulfuric acid (1.06 mL, 1.1 eq.) was added to the solution at 20° C. The reaction mixture was heated to reflux temperature for 2 hours during which a turbid solution was formed. Then, the solution was cooled to room temp...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
ClCCl
null
16
O=S(=O)(O)O>ClCCl>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-32168cbcc4634df6ae32c9a9b1ce0afe
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
C1(=CC=CC=C1)C
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
82
[{"value": 82.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
16
HOUR
Clopidogrel base (4.29 g, 1 eq.) was dissolved in toluene (33.8 mL). Eighty percent aqueous sulfuric acid (1.04 mL, 1.1 eq.) was added to the solution at 20° C. The reaction mixture was heated to reflux temperature for 3 hours. Then, the solution was cooled to room temperature and stirred at this temperature for an add...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
C1(=CC=CC=C1)C
null
16
O=S(=O)(O)O>C1(=CC=CC=C1)C>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-7b9e0f91bee940479df50ee03db26c63
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
C(Cl)(Cl)Cl
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
56
[{"value": 56.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
Clopidogrel base (4.24 g, leq.) was dissolved in chloroform (33.4 mL). Eighty percent aqueous sulfuric acid (0.62 mL, 0.66 eq.) was added to the solution at 20° C. The reaction mixture was heated to reflux temperature for 2 hours during which a precipitate was formed. Then, the solution was cooled to room temperature a...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
C(Cl)(Cl)Cl
null
null
O=S(=O)(O)O>C(Cl)(Cl)Cl>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-19e8796c29e342a39995c84f04d3a2f2
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
C(Cl)(Cl)Cl
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
88
[{"value": 88.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
16
HOUR
Clopidogrel base (4.37 g, leq.) was dissolved in chloroform (34.5 mL). Eighty percent aqueous sulfuric acid (1.06 ml, 1.1 eq.) was added to the solution at 20° C. The reaction mixture was heated to reflux temperature for 2 hours during which a precipitate was formed. Then, the solution was cooled to room temperature an...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
C(Cl)(Cl)Cl
null
16
O=S(=O)(O)O>C(Cl)(Cl)Cl>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d3b54ffe4ed14f94b2630339c1c540ca
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
C(C)(=O)OCC
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
49
[{"value": 49.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
16
HOUR
Clopidogrel base (4.03 g, 1 eq.) was dissolved in ethyl acetate (31.8 mL). Eighty percent aqueous sulfuric acid (0.59 mL, 0.66 eq.) was added to the solution at 20° C. The reaction mixture was heated to reflux temperature for 3 hours during which a sticky precipitate was formed. Then, the solution was cooled to room te...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
C(C)(=O)OCC
null
16
O=S(=O)(O)O>C(C)(=O)OCC>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-47881f4596bd4cffabd3e61aec361380
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
C(C)(=O)OCC
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
66
[{"value": 66.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
Clopidogrel base (5.31 g, leq.) was dissolved in ethyl acetate (41.9 mL). Eighty percent aqueous sulfuric acid (1.29 mL, 1.1 eq.) was added to the solution at 20° C. The reaction mixture was heated to reflux temperature for 2 hours during which a massive precipitate was formed. Then, the solution was cooled to room tem...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
C(C)(=O)OCC
null
3
O=S(=O)(O)O>C(C)(=O)OCC>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0b818c555a26422ca7684099ad68aa00
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
C(C)(C)(C)OC
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
52
[{"value": 52.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
Clopidogrel base (4.39 g, leq.) was dissolved in tert-butylmethyl ether (MTBE) (34.6 ml). Eighty percent aqueous sulfuric acid (0.64 ml, 0.66 eq.) was added to the solution at 20° C. The reaction mixture was heated to reflux temperature for 3 hours during which a sticky precipitate was formed. Then, the solution was co...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
C(C)(C)(C)OC
null
2
O=S(=O)(O)O>C(C)(C)(C)OC>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-86d7792015834df69da12ccbb57a5238
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
O1CCOCC1
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
48
[{"value": 48.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
Clopidogrel base (4.17 g, leq.) was dissolved in 1,4-Dioxane (32.9 mL). Eighty percent aqueous sulfuric acid (0.61 ml, 0.66 eq.) was added to the solution at 20° C. The reaction mixture was heated to reflux temperature for 2 hours during which a massive precipitate was formed. Then, the solution was cooled to room temp...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
O1CCOCC1
null
2
O=S(=O)(O)O>O1CCOCC1>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b576c48cd9f74a05ae8ae061f693d5bb
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
CC(=O)C
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
78
[{"value": 78.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
1.5
HOUR
Clopidogrel base (3.42 g) was dissolved in acetone (27 mL). Aqueous sulfuric acid (20%, 4.57 mL) was added to the solution at 20° C. The reaction mixture was heated to reflux temperature for 2 hours. The solution was cooled to room temperature and stirred at this temperature for additional 1.5 hours. Then the solvent w...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
CC(=O)C
null
1.5
O=S(=O)(O)O>CC(=O)C>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-228f057bae954144b16d8660a2593903
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
CC(=O)C
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
82
[{"value": 82.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
Clopidogrel base (2.88 g) was dissolved in acetone (23 mL). Aqueous sulfuric acid (20%, 2.56 mL) was added to the solution at 20° C. The reaction mixture was heated to reflux temperature for 2 hours. The solution was cooled to room temperature and stirred at this temperature for an additional 2 hours. Then the solvent ...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
CC(=O)C
null
2
O=S(=O)(O)O>CC(=O)C>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-42f2b151a28f46b786c53e833f1688e2
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
C(C)(C)(C)OC.C(C)O
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
56
[{"value": 56.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
Clopidogrel base (3.85 g) was dissolved in absolute ethanol (30.4 mL). Eighty percent aqueous sulfuric acid (0.56 mL) was added to the solution. The reaction mixture was heated to reflex temperature for 2 hours. Then, the solution was cooled to room temperature and the solvent was evaporated to dryness under reduced pr...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
C(C)(C)(C)OC.C(C)O
null
null
O=S(=O)(O)O>C(C)(C)(C)OC.C(C)O>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ac280c140bb948b98b2c2e9fe6e65d9d
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
C(CCC)O.C(C)(C)(C)OC
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
60
[{"value": 60.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
Clopidogrel base (4.28 g) was dissolved in 1-butanol (16.9 ml). Eighty percent aqueous sulfuric acid (0.63 ml) was added to the solution at 20° C. The reaction mixture was heated to reflux temperature for 2 hours. Then, the solution was cooled to room temperature and the solvent was evaporated to dryness under reduced ...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
C(CCC)O.C(C)(C)(C)OC
null
null
O=S(=O)(O)O>C(CCC)O.C(C)(C)(C)OC>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e29829a0079844738f99dbb5e4014801
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
C(C)(C)O
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
71
[{"value": 71.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
Clopidogrel base (2.96 g) was dissolved in isopropanol (45 mL). Aqueous sulfuric acid (98%, 0.50 ml) was added to the solution at 20° C. The reaction mixture was heated to reflux temperature for 2 hours. Then, the solution was cooled to room temperature and stirred at this temperature for an additional 2 hours to obtai...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
C(C)(C)O
null
2
O=S(=O)(O)O>C(C)(C)O>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-85ed19cd08aa4fefbfe32f1b899cbf4e
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
C(C)(C)O
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
80
[{"value": 80.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
Clopidogrel base (2.91 g) was dissolved in isopropanol (IPA) (44 ml). Ninety eight percent aqueous sulfuric acid (0.32 ml) was added to the solution at 20° C. The reaction mixture was heated to reflux temperature for 2 hours. Then, the solution was cooled to room temperature and stirred at this temperature for an addit...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
C(C)(C)O
null
2
O=S(=O)(O)O>C(C)(C)O>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-1e34d4f4189c4b309cb8319fcb6e162d
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
C(C)(C)O
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
58
[{"value": 58.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
2.5
HOUR
Clopidogrel base (2.93 g) was dissolved in isopropanol (45 ml). Sixty percent aqueous sulfuric acid (0.99 mL) was added to the solution at 20° C. The reaction mixture was heated to reflux temperature for 2 hours. Then, the solution was cooled to room temperature and stirred at this temperature for an additional 2.5 hou...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
C(C)(C)O
null
2.5
O=S(=O)(O)O>C(C)(C)O>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-92dc22b5901547448a58e8410fb8ef3b
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
C(C)(C)O
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
24
[{"value": 24.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
Clopidogrel base (2.98 g) was dissolved in isopropanol (45 mL). Sixty percent aqueous sulfuric acid (0.67 ml) was added to the solution at 20° C. The reaction mixture was heated to reflux temperature for 2 hours. Then, the solution was cooled to room temperature and stirred at this temperature for additional 2 hours to...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
C(C)(C)O
null
2
O=S(=O)(O)O>C(C)(C)O>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0f2df6e7a6be40a9a2b6c14fa466eb0c
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
C(C)(C)O
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
40
[{"value": 40.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
3.5
HOUR
Clopidogrel base (2.85 g) was dissolved in isopropanol (43 mL). Forty percent aqueous sulfuric acid (1.67 mL) was added to the solution at 20° C. The reaction mixture was heated to reflex temperature for 2 hours. Then, the solution was cooled to room temperature and stirred at this temperature for additional 3.5 hours ...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
C(C)(C)O
null
3.5
O=S(=O)(O)O>C(C)(C)O>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b809176d5b3942438dee231ec3fc784f
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
C(C)(C)O
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
13
[{"value": 13.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
3.5
HOUR
Clopidogrel base (2.95 g) was dissolved in isopropanol (45 ml). Forty percent aqueous sulfuric acid (1.15 mL) was added to the solution at 20° C. The reaction mixture was heated to reflux temperature for 2 hours. Then, the solution was cooled to room temperature and stirred at this temperature for an additional 3.5 hou...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
C(C)(C)O
null
3.5
O=S(=O)(O)O>C(C)(C)O>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-54d89a4f8a55464d88343966b45eea5b
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
C(C)(C)O
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
33
[{"value": 33.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
5
HOUR
Clopidogrel base (2.89 g) was dissolved in isopropanol (44 mL). Eighty percent aqueous sulfuric acid (0.42 mL) was added to the solution at 20° C. The reaction mixture was heated to reflux temperature for 2 hours. The solution was cooled to room temperature and stirred at this temperature for an additional 5 hours. The...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
C(C)(C)O
null
5
O=S(=O)(O)O>C(C)(C)O>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-8ac6d6779bed4433a60a395433fd4f17
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
C(C)(C)O
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
84
[{"value": 84.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
1.5
HOUR
Clopidogrel base (2.96 g) was dissolved in isopropanol (IPA) (45 mL). Eighty percent aqueous sulfuric acid (0.65 mL) was added to the solution at 20° C. The reaction mixture was heated to reflux temperature for 2 hours. Then, the solution was cooled to room temperature and stirred at this temperature for an additional ...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
C(C)(C)O
null
1.5
O=S(=O)(O)O>C(C)(C)O>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-79a88380673f4a60829378d6d2f0f878
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O.COC(C)(C)C>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
CC(CC)O
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
87
[{"value": 87.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
Clopidogrel base (2.98 g) was dissolved in 2-butanol (23 mL). Ninety eight percent aqueous sulfuric acid (0.50 mL) was added to the solution at 20° C. The reaction mixture was heated to reflux temperature for 2 hours. The solution was cooled to room temperature and stirred at this temperature for an additional 3 hours....
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
CC(CC)O
null
3
O=S(=O)(O)O>CC(CC)O>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e10d3fa053c0492dba9696b145cfbfd8
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O.C(C)OCC>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
CC(CC)O
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
55
[{"value": 55.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
1.5
HOUR
Clopidogrel base (2.94 g) was dissolved in 2-butanol (23 mL). Ninety eight percent aqueous sulfuric acid (0.43 mL) was added to the solution at 20° C. The reaction mixture was heated to reflex temperature for 2 hours. The solution was cooled to room temperature and stirred at this temperature for additional 1.5 hours. ...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
CC(CC)O
null
1.5
O=S(=O)(O)O>CC(CC)O>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-70a1d2b862e2446f9dbfd0405e0a6f96
O=S(=O)(O)O>>O=S(=O)(O)O
COC(=O)[C@H](C=1C=CC=CC1Cl)N2CCC3=C(C=CS3)C2.S(O)(O)(=O)=O.CC(C)(C)OC>>COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O
[O:22]=[S:23](=[O:24])([OH:25])[OH:26]>>[O:22]=[S:23](=[O:24])([OH:25])[OH:26]
O=S(=O)(O)O
O=S(=O)(O)O
null
null
C(CC)O
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
null
null
69
[{"value": 69.0, "product": "COC(=O)[C@H](C1=CC=CC=C1Cl)N2CCC3=C(C2)C=CS3.OS(=O)(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
16
HOUR
Clopidogrel base (2.86 g, 1 eq.) was dissolved in 1-Propanol (22.6 mL). Eighty percent aqueous sulfuric acid (0.59 mL, 0.66 eq.) was added to the solution at 20° C. The reaction mixture was heated to reflux temperature for 2 hours. Then, the solution was cooled to room temperature and stirred at this temperature for ad...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
null
null
C(CC)O
null
16
O=S(=O)(O)O>C(CC)O>O=S(=O)(O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d4226d2232fe4b14a19c35ee9bd4e93f
Brc1cnc2ccccc2c1.C#CCO>>OCC#Cc1cnc2ccccc2c1
BrC=1C=NC2=CC=CC=C2C1.C(C#C)O.C(C)N(CC)CC.C(C)N(CC)CC>>N1=CC(=CC2=CC=CC=C12)C#CCO
Br[c:5]1[cH:6][n:7][c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]2[cH:14]1.[OH:1][CH2:2][C:3]#[CH:4]>>[OH:1][CH2:2][C:3]#[C:4][c:5]1[cH:6][n:7][c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]2[cH:14]1
Brc1cnc2ccccc2c1.C#CCO
OCC#Cc1cnc2ccccc2c1
null
[Cu]I
C(=O)(O)[O-].[Na+]
C-C Coupling
Sonogashira alkyne_aryl halide
1e174391e4a252d3fd1450e5e0322e210429c2a497011bc6a30357bb5bc3eef3
305eca0fd2975da49e7f69e4edfb9dc1cbce82513954bc5a73be3289e70e5f76
c1ccc2ncccc2c1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[#7;a:5]:[c:6]:1.[C:7]-[C:8]#[CH;D1;+0:9]>>[C:7]-[C:8]#[C;H0;D2;+0:9]-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[#7;a:5]:[c:6]:1
88.3
[{"value": 88.3, "product": "N1=CC(=CC2=CC=CC=C12)C#CCO", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
To a dry 2-L three-necked flask previously purged with nitrogen was charged 3-bromoquinoline (118.77 g, 570 mmol), propargyl alcohol (71.9 g, 1.28 mol, 2.25 equiv), triethylamine (1500 mL), copper(I) iodide (3.62, 19 mmol, 0.033 equiv) and dichlorobis(triphenyl-phosphine) palladium(II) (6.67 g, 9.5 mmol). The mixture w...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Alkyne
Alkyne
c1ccc2ncccc2c1
c1ccc2ncccc2c1
c1ccc2ncccc2c1
HBr
[Cu]I.C(=O)(O)[O-].[Na+]
null
null
Brc1cnc2ccccc2c1.C#CCO>[Cu]I.C(=O)(O)[O-].[Na+]>OCC#Cc1cnc2ccccc2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-47b9e37a882e47ecb16f8a0de6198a24
OCC#Cc1cnc2ccccc2c1>>OC/C=C/c1cnc2ccccc2c1
[H-].COCCO[Al+]OCCOC.[Na+].[H-].N1=CC(=CC2=CC=CC=C12)C#CCO>>N1=CC(=CC2=CC=CC=C12)/C=C/CO
[OH:1][CH2:2][C:3]#[C:4][c:5]1[cH:6][n:7][c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]2[cH:14]1>>[OH:1][CH2:2]/[CH:3]=[CH:4]/[c:5]1[cH:6][n:7][c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]2[cH:14]1
OCC#Cc1cnc2ccccc2c1
OC/C=C/c1cnc2ccccc2c1
null
null
C1CCOC1
Reduction
Hydrogenation (triple to double)
2bb8d5b532a2781e0a7c069a5cd3e8a7e8d44660c0ec1d9e17c04d8ba2cb383b
1990560e9c55934bde8ca0feaed9c61d80f37f94f0cf240a9929dc374d0a33aa
c1ccc2ncccc2c1
[O;D1;H1:1]-[C:2]-[C;H0;D2;+0:3]#[C;H0;D2;+0:4]-[c:5](:[c:6]):[c:7]:[#7;a:8]:[c:9]>>[O;D1;H1:1]-[C:2]/[CH;D2;+0:3]=[CH;D2;+0:4]/[c:5](:[c:6]):[c:7]:[#7;a:8]:[c:9]
null
[]
null
null
1
HOUR
To a dry, jacketed 250-mL three-necked round-bottom flask was charged sodium bis(2-methoxyethoxy)aluminum hydride (Red-Al, 70% wt. solution in toluene, 11.0 g, 38.1 mmol, 1.39 eq) and anhydrous THF (20 mL). To this precooled (0–2° C.) and magnetically stirred solution was added a THF (50 mL) solution of the 3-(3-quinol...
10.6084/m9.figshare.5104873.v1
null
Alkyne
null
null
null
c1ccc2ncccc2c1
null
C1CCOC1
null
1
OCC#Cc1cnc2ccccc2c1>C1CCOC1>OC/C=C/c1cnc2ccccc2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-ad72a4378b3b4b24a50d107af25b2797
CC(C)(C)OC(=O)OC(=O)OC(C)(C)C>>CC(C)(C)OC(=O)[O-]
C(C)(=O)OCC.CCCCCCC.[OH-].[Na+].N1=CC(=CC2=CC=CC=C12)C=CCO.C(=O)(OC(C)(C)C)OC(=O)OC(C)(C)C>>N1=CC(=CC2=CC=CC=C12)C=CCO.C(OC(C)(C)C)([O-])=O
CC(C)(C)OC(=O)[O:8][C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[O-:8]
CC(C)(C)OC(=O)OC(=O)OC(C)(C)C
CC(C)(C)OC(=O)[O-]
null
S(=O)(=O)(O)[O-].C(CCC)[N+](CCCC)(CCCC)CCCC
C(Cl)Cl
Miscellaneous
OtherReaction
ed733215f442ec38ffb8ac8e3ce0777b9978fcccda2fe55610efa73305a71ba0
5ef46932d9a1fe5669b3d06c14ca4f5627ea1d329652fc6287924421b334d6e3
null
C-C(-C)(-C)-O-C(=O)-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#8:4]-[C:5](-[C;D1;H3:6])(-[C;D1;H3:7])-[C;D1;H3:8]>>[C;D1;H3:6]-[C:5](-[C;D1;H3:7])(-[C;D1;H3:8])-[#8:4]-[C:2](-[O-;H0;D1:1])=[O;D1;H0:3]
null
[]
null
null
null
null
To a 500-mL three-necked round-bottom flask equipped with an overhead mechanical stirrer was charged 3-(3-quinolyl)-2-propen-1-ol (13.03 g, 70.43 mmol) as a mixture of cis- and trans-isomers (81% cis, and 19% trans), di-tert butyl dicarbonate (16.91 g, 77.48 mmol, 1.11 equiv), tetra n-butylammonium hydrogen sulfate (74...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Carbonic Ester.Carbonic Ester.Boc
Carbonic Acid
null
null
null
HO-
S(=O)(=O)(O)[O-].C(CCC)[N+](CCCC)(CCCC)CCCC.C(Cl)Cl
null
null
CC(C)(C)OC(=O)OC(=O)OC(C)(C)C>S(=O)(=O)(O)[O-].C(CCC)[N+](CCCC)(CCCC)CCCC.C(Cl)Cl>CC(C)(C)OC(=O)[O-]
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-044e5cc4fd5e4afc9a7e9c694199cff7
CC(C)(C)OC(=O)OC(=O)OC(C)(C)C>>CC(C)(C)OC(=O)[O-]
N1=CC(=CC2=CC=CC=C12)C#CCO.C(=O)(OC(C)(C)C)OC(=O)OC(C)(C)C.[OH-].[Na+]>>N1=CC(=CC2=CC=CC=C12)C#CCO.C(C)(C)(C)OC([O-])=O
CC(C)(C)OC(=O)[O:8][C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[O-:8]
CC(C)(C)OC(=O)OC(=O)OC(C)(C)C
CC(C)(C)OC(=O)[O-]
null
null
O.C(Cl)Cl
Miscellaneous
OtherReaction
ed733215f442ec38ffb8ac8e3ce0777b9978fcccda2fe55610efa73305a71ba0
5ef46932d9a1fe5669b3d06c14ca4f5627ea1d329652fc6287924421b334d6e3
null
C-C(-C)(-C)-O-C(=O)-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#8:4]-[C:5](-[C;D1;H3:6])(-[C;D1;H3:7])-[C;D1;H3:8]>>[C;D1;H3:6]-[C:5](-[C;D1;H3:7])(-[C;D1;H3:8])-[#8:4]-[C:2](-[O-;H0;D1:1])=[O;D1;H0:3]
null
[]
null
null
4
HOUR
To a dry 1-L three-necked round-bottom flask equipped with a nitrogen inlet and overhead stirrer was charged 3-(3-quinolyl)-2-propyn-1-ol (15.81 g, 86.39 mmol), di-tert-butyl dicarbonate (22.48 g, 103 mmol, 1.19 equiv), n-tetrabutyl ammonium hydrogen sulfate (0.86 g, 2.54 mmol, 0.029 equiv) and methylene chloride (300 ...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Carbonic Ester.Carbonic Ester.Boc
Carbonic Acid
null
null
null
HO-
O.C(Cl)Cl
null
4
CC(C)(C)OC(=O)OC(=O)OC(C)(C)C>O.C(Cl)Cl>CC(C)(C)OC(=O)[O-]
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b409aa7fda1e49bbb7bfb0b9464b3638
OCC#Cc1cnc2ccccc2c1>>OCC=Cc1cnc2ccccc2c1
N1=CC(=CC2=CC=CC=C12)C#CCO.C(C)(C)(C)OC([O-])=O>>N1=CC(=CC2=CC=CC=C12)C=CCO.C(C)(C)(C)OC([O-])=O
[OH:9][CH2:10][C:11]#[C:12][c:13]1[cH:14][n:15][c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[cH:22]1>>[OH:9][CH2:10][CH:11]=[CH:12][c:13]1[cH:14][n:15][c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]2[cH:22]1
OCC#Cc1cnc2ccccc2c1
OCC=Cc1cnc2ccccc2c1
null
[Pd].[Pd].CC(=O)[O-].CC(=O)[O-].[Pb+2]
C(C)(C)O
Reduction
Hydrogenation (triple to double)
2bb8d5b532a2781e0a7c069a5cd3e8a7e8d44660c0ec1d9e17c04d8ba2cb383b
1990560e9c55934bde8ca0feaed9c61d80f37f94f0cf240a9929dc374d0a33aa
c1ccc2ncccc2c1
[O;D1;H1:1]-[C:2]-[C;H0;D2;+0:3]#[C;H0;D2;+0:4]-[c:5](:[c:6]):[c:7]:[#7;a:8]:[c:9]>>[O;D1;H1:1]-[C:2]-[CH;D2;+0:3]=[CH;D2;+0:4]-[c:5](:[c:6]):[c:7]:[#7;a:8]:[c:9]
null
[]
null
null
null
null
To a 250-mL single-necked round-bottom flask was charged the 3-(3-quinolyl)-2-propyn-1-ol t-butyl carbonate (1.52 g, 5.37 mmol), isopropanol (30 mL) and 5% palladium on calcium carbonate poisoned with lead (Lindlar's catalyst, 75 mg, 0.049 equiv). The suspension was stirred (rapidly) magnetically and the atmosphere abo...
10.6084/m9.figshare.5104873.v1
null
Alkyne
null
null
null
c1ccc2ncccc2c1
null
[Pd].[Pd].CC(=O)[O-].CC(=O)[O-].[Pb+2].C(C)(C)O
null
null
OCC#Cc1cnc2ccccc2c1>[Pd].[Pd].CC(=O)[O-].CC(=O)[O-].[Pb+2].C(C)(C)O>OCC=Cc1cnc2ccccc2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f83c87bc9b8c4febad52cb8f24326a21
Brc1cnc2ccccc2c1.C=CC(=O)OCC>>CCOC(=O)C=Cc1cnc2ccccc2c1
CN(C=O)C.BrC=1C=NC2=CC=CC=C2C1.C(C=C)(=O)OCC.C([O-])(O)=O.[Na+].BrC=1C=NC2=CC=CC=C2C1>>N1=CC(=CC2=CC=CC=C12)C=CC(=O)OCC
Br[c:8]1[cH:9][n:10][c:11]2[cH:12][cH:13][cH:14][cH:15][c:16]2[cH:17]1.[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]=[CH2:7]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]=[CH:7][c:8]1[cH:9][n:10][c:11]2[cH:12][cH:13][cH:14][cH:15][c:16]2[cH:17]1
Brc1cnc2ccccc2c1.C=CC(=O)OCC
CCOC(=O)C=Cc1cnc2ccccc2c1
null
[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC.C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-]
C(C)(=O)OCC
C-C Coupling
Heck terminal vinyl
a87d881b4c1880689693d296001ccd251ba98c523b412e68ce627333ac531f30
4b186811a4930853b446d93d9faa39b267bddb9ce0b8021bda5c5a3b2bc69f0b
c1ccc2ncccc2c1
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[#7;a:5]:[c:6]:1.[C:7]-[#8:8]-[C:9](=[O;D1;H0:10])-[C:11]=[CH2;D1;+0:12]>>[C:7]-[#8:8]-[C:9](=[O;D1;H0:10])-[C:11]=[CH;D2;+0:12]-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[#7;a:5]:[c:6]:1
65
[{"value": 65.0, "product": "N1=CC(=CC2=CC=CC=C12)C=CC(=O)OCC", "details": "PERCENTYIELD", "is_desired": false}]
90
CELSIUS
30
MINUTE
The 3-bromoquinoline (300 g, 1.44 mmol), ethyl acrylate (168 g, 1.68 mmol), palladium(II) acetate (32.3 g, 144 mmol), tetrabutylammonium bromide (478 g 1.44 mol), and sodium bicarbonate (483.9 g, 5.76 mol) were combined in a 5-L round-bottom flask with overhead stirring and 3 L dimethyl formamide (anhydrous). The react...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Vinyl
null
c1ccc2ncccc2c1
c1ccc2ncccc2c1
c1ccc2ncccc2c1
HBr
[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC.C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].C(C)(=O)OCC
90
0.5
Brc1cnc2ccccc2c1.C=CC(=O)OCC>[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC.C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].C(C)(=O)OCC>CCOC(=O)C=Cc1cnc2ccccc2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-c892151205ac4c359da3777a59ad165c
O=C([O-])C=Cc1cnc2ccccc2c1>>OCC=Cc1cnc2ccccc2c1
N1=CC(=CC2=CC=CC=C12)C=CC(=O)[O-].[H-].C(C(C)C)[Al+]CC(C)C>>N1=CC(=CC2=CC=CC=C12)C=CCO
O=[C:2]([O-:1])[CH:3]=[CH:4][c:5]1[cH:6][n:7][c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]2[cH:14]1>>[OH:1][CH2:2][CH:3]=[CH:4][c:5]1[cH:6][n:7][c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]2[cH:14]1
O=C([O-])C=Cc1cnc2ccccc2c1
OCC=Cc1cnc2ccccc2c1
null
null
C(Cl)Cl
Reduction
OtherReaction
3ee00ae8302f5a9cabfd43f47c90c2bc696c7c0e2b77ca13873c453d0520692e
c2c13922fe3c9358e6ba38897f2383764691ea247b267e6643408d03716a3879
c1ccc2ncccc2c1
O=[C;H0;D3;+0:1](-[O-;H0;D1:2])-[C:3]=[C:4]-[c:5]:[c:6]:[#7;a:7]>>[#7;a:7]:[c:6]:[c:5]-[C:4]=[C:3]-[CH2;D2;+0:1]-[OH;D1;+0:2]
62
[{"value": 62.0, "product": "N1=CC(=CC2=CC=CC=C12)C=CCO", "details": "PERCENTYIELD", "is_desired": false}, {"value": 61.7, "product": "N1=CC(=CC2=CC=CC=C12)C=CCO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-57
CELSIUS
30
MINUTE
The 3-(3-quinolyl)-2-propenoate (141 g, 0.621 moles) was dissolved in 2.0 L anhydrous methylene chloride in a 5-L round-bottom flask with overhead stirring and cooled to −57° C. with isopropanol/dry ice bath. Diisobutylaluminum hydride (1.55 L, 1.0 M in methylene chloride) was added in a slow stream, keeping the temper...
10.6084/m9.figshare.5104873.v1
null
null
Primary alcohol
null
null
c1ccc2ncccc2c1
Other
C(Cl)Cl
-57
0.5
O=C([O-])C=Cc1cnc2ccccc2c1>C(Cl)Cl>OCC=Cc1cnc2ccccc2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-108b40c914184cc48154e402484aabce
CC(C)(C)OC(=O)OC(=O)OC(C)(C)C.O=Cc1cc2ccccc2nc1I>>C=CC(O)c1cnc2ccccc2c1.CC(C)(C)OC(=O)[O-]
C(=O)(OC(C)(C)C)OC(=O)OC(C)(C)C.IC1=NC2=CC=CC=C2C=C1C=O.C(=C)[Mg]Br.[Cl-].[NH4+].[Li+].CCC[CH2-]>>N1=CC(=CC2=CC=CC=C12)C(C=C)O.C(C)(C)(C)OC([O-])=O
CC(C)(C)OC(=O)[O:22][C:20]([O:19][C:16]([CH3:15])([CH3:17])[CH3:18])=[O:21].I[c:6]1[c:5]([CH:3]=[O:4])[cH:14][c:13]2[c:8]([n:7]1)[cH:9][cH:10][cH:11][cH:12]2>>[CH2:1]=[CH:2][CH:3]([OH:4])[c:5]1[cH:6][n:7][c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]2[cH:14]1.[CH3:15][C:16]([CH3:17])([CH3:18])[O:19][C:20](=[O:21])[O-:22]
CC(C)(C)OC(=O)OC(=O)OC(C)(C)C.O=Cc1cc2ccccc2nc1I
C=CC(O)c1cnc2ccccc2c1.CC(C)(C)OC(=O)[O-]
null
null
CC(C)(C)OC.C1CCOC1
C-C Coupling
OtherReaction
c37b84f8c11ce4454b903ce99294ae1ca011988fca379ee616427f283b4bed0c
19cb132516618b7155a282cb13664293728ad4558cd3dc48c98aa6ff43004e7a
c1ccc2ncccc2c1
C-C(-C)(-C)-O-C(=O)-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#8:4]-[C:5](-[C;D1;H3:6])(-[C;D1;H3:7])-[C;D1;H3:8].I-[c;H0;D3;+0:9](:[#7;a:10]:[c:11]):[c:12](-[CH;D2;+0:13]=[O;H0;D1;+0:14]):[c:15]>>[C;D1;H2:16]=[C:17]-[CH;D3;+0:13](-[OH;D1;+0:14])-[c:12](:[c:15]):[cH;D2;+0:9]:[#7;a:10]:[c:11].[C;D1;H3:6]-[C:5](-[C;D1;H3:7])(-...
null
[]
null
null
1
HOUR
To a solution of 2-iodo-3-quinoline carboxaldehyde (3 g, 10.6 mmol) in THF (25 ml) at −5° C., vinylmagnesium bromide (1 M solution, 10. 8 ml, 10.8 mmol) was added. It was stirred at that temperature until the starting material disappears, which takes about one hour. N-butyllithium (8.5 ml, 2.5 M soln, 21.2 mmol) was ad...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Anhydride.Aldehyde.Carbonic Ester.Carbonic Ester.Boc
Carbonic Acid.Secondary alcohol.Vinyl
c1ccc2ncccc2c1
c1ccc2ncccc2c1
c1ccc2ncccc2c1
HI
CC(C)(C)OC.C1CCOC1
null
1
CC(C)(C)OC(=O)OC(=O)OC(C)(C)C.O=Cc1cc2ccccc2nc1I>CC(C)(C)OC.C1CCOC1>C=CC(O)c1cnc2ccccc2c1.CC(C)(C)OC(=O)[O-]
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-68927fb1a4ea43b9a8e0239686c36b4d
CC=O.O=Cc1cnc2ccccc2c1>>O=CC=Cc1cnc2ccccc2c1
C(C)(=O)OC(C)=O.[OH-].[Na+].N1=CC(=CC2=CC=CC=C12)C=O.C(C)=O.C(C)(=O)OC>>N1=CC(=CC2=CC=CC=C12)C=CC=O
[O:1]=[CH:2][CH3:3].O=[CH:4][c:5]1[cH:6][n:7][c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]2[cH:14]1>>[O:1]=[CH:2][CH:3]=[CH:4][c:5]1[cH:6][n:7][c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]2[cH:14]1
CC=O.O=Cc1cnc2ccccc2c1
O=CC=Cc1cnc2ccccc2c1
null
null
O.CO
C-C Coupling
OtherReaction
154f038b7f5648ae5349abff8a924c982177f620bdfb6a2f53d7ca0fce37c68d
3174a51604157c488f07402e36f994f716989b8fc10687ee243713b4cfbdb11a
c1ccc2ncccc2c1
O=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4]:[#7;a:5]:[c:6].[CH3;D1;+0:7]-[C:8]=[O;D1;H0:9]>>[O;D1;H0:9]=[C:8]-[CH;D2;+0:7]=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4]:[#7;a:5]:[c:6]
null
[]
-10
CELSIUS
30
MINUTE
To a 500-mL round-bottom flask, equipped with mechanical stirrer, dropping funnel and temperature bath was charged 30.9 g (0.2 mol) quinoline 3-carboxaldehyde and acetaldehyde (50 mL). The mixture was cooled to −10° C. and a solution of sodium hydroxide (500 mg) in methanol (8 mL) was added dropwise keeping the tempera...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Aldehyde
Aldehyde
null
null
c1ccc2ncccc2c1
HO-
O.CO
-10
0.5
CC=O.O=Cc1cnc2ccccc2c1>O.CO>O=CC=Cc1cnc2ccccc2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0d067d67eb604ce780e28de10f9cd37b
O=CC=Cc1cnc2ccccc2c1>>OCC=Cc1cnc2ccccc2c1
[Cl-].[NH4+].[BH4-].[Na+].N1=CC(=CC2=CC=CC=C12)C=CC=O.C(C)(=O)OC(C)C>>N1=CC(=CC2=CC=CC=C12)C=CCO
[O:1]=[CH:2][CH:3]=[CH:4][c:5]1[cH:6][n:7][c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]2[cH:14]1>>[OH:1][CH2:2][CH:3]=[CH:4][c:5]1[cH:6][n:7][c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]2[cH:14]1
O=CC=Cc1cnc2ccccc2c1
OCC=Cc1cnc2ccccc2c1
null
null
CO
Reduction
Reduction of aldehydes and ketones to alcohols
e7895795cd3f75445716c94697823c5929dcd4b5344525875fe75d36bca2f9d7
21bb81d5469aaaca71ab12c186bea4016451717fad8780cf288858a7d8fbc55a
c1ccc2ncccc2c1
[#7;a:1]:[c:2]:[c:3]-[C:4]=[C:5]-[CH;D2;+0:6]=[O;H0;D1;+0:7]>>[#7;a:1]:[c:2]:[c:3]-[C:4]=[C:5]-[CH2;D2;+0:6]-[OH;D1;+0:7]
65.4
[{"value": 65.4, "product": "N1=CC(=CC2=CC=CC=C12)C=CCO", "details": "PERCENTYIELD", "is_desired": false}, {"value": 65.3, "product": "N1=CC(=CC2=CC=CC=C12)C=CCO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
23
CELSIUS
90
MINUTE
A mixture of 3-(3-quinolyl)propenal (10 g, 54.6 mmol) in methanol (50 mL) was cooled to 0° C. and to this mixture, sodium borohydride (1.03 g, 27 mmol) was charged in small portions keeping the temperature below 10° C. After the addition was complete, the mixture was stirred at 23° C. for 90 min. until the reaction was...
10.6084/m9.figshare.5104873.v1
null
Aldehyde
Primary alcohol
null
null
c1ccc2ncccc2c1
null
CO
23
1.5
O=CC=Cc1cnc2ccccc2c1>CO>OCC=Cc1cnc2ccccc2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-977be506a4914aa1a39f7b8627dcf552
O=C(Cl)N(C1CCCCC1)C1CCCCC1.OCC#Cc1cnc2ccccc2c1>>O=C(OCC#Cc1cnc2ccccc2c1)N(C1CCCCC1)C1CCCCC1
[NH4+].[Cl-].CC(C)([O-])C.[K+].N1=CC(=CC2=CC=CC=C12)C#CCO.C1(CCCCC1)N(C(=O)Cl)C1CCCCC1>>C1(CCCCC1)N(C(=O)OCC#CC=1C=NC2=CC=CC=C2C1)C1CCCCC1
Cl[C:2](=[O:1])[N:17]([CH:18]1[CH2:19][CH2:20][CH2:21][CH2:22][CH2:23]1)[CH:24]1[CH2:25][CH2:26][CH2:27][CH2:28][CH2:29]1.[OH:3][CH2:4][C:5]#[C:6][c:7]1[cH:8][n:9][c:10]2[cH:11][cH:12][cH:13][cH:14][c:15]2[cH:16]1>>[O:1]=[C:2]([O:3][CH2:4][C:5]#[C:6][c:7]1[cH:8][n:9][c:10]2[cH:11][cH:12][cH:13][cH:14][c:15]2[cH:16]1)[N...
O=C(Cl)N(C1CCCCC1)C1CCCCC1.OCC#Cc1cnc2ccccc2c1
O=C(OCC#Cc1cnc2ccccc2c1)N(C1CCCCC1)C1CCCCC1
null
null
CC(C)(C)OC.C1CCOC1
Protection
Schotten-Baumann to ester
597fa7ba4ca169ec9e1d3b8730fbab27757ccde00143c31019a679c09b7b2b7f
562b6a5118cb63cbe5ff058f35135dc3f085de8b8ec7fa4ac4de518324eb826a
O=C(OCC#Cc1cnc2ccccc2c1)N(C1CCCCC1)C1CCCCC1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#7:3](-[C:4])-[C:5].[#7;a:6]:[c:7]:[c:8]-[C:9]#[C:10]-[C:11]-[OH;D1;+0:12]>>[#7;a:6]:[c:7]:[c:8]-[C:9]#[C:10]-[C:11]-[O;H0;D2;+0:12]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#7:3](-[C:4])-[C:5]
null
[]
0
CELSIUS
2
HOUR
To a dry three-necked round-bottom flask equipped with nitrogen inlet and overhead stirrer was charged 3-(3-quinolyl)-2-propyn-1-ol (1 g, 5.4 mmol) in THF (10 ml) and the solution was cooled to 0° C. Potassium t-butoxide (0.67 g, 5.9 mmol) was then added followed by dicyclohexylcarbamoyl chloride (1.32 g, 5.4 mmol). Th...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Tertiary amide.Primary alcohol
Carbamic ester
null
null
c1ccc2ncccc2c1.C1CCCCC1.C1CCCCC1
HCl
CC(C)(C)OC.C1CCOC1
0
2
O=C(Cl)N(C1CCCCC1)C1CCCCC1.OCC#Cc1cnc2ccccc2c1>CC(C)(C)OC.C1CCOC1>O=C(OCC#Cc1cnc2ccccc2c1)N(C1CCCCC1)C1CCCCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d58dd4469bd14d00b3e47bcff1963e73
O=C(Cl)N(c1ccccc1)c1ccccc1.OCC#Cc1cnc2ccccc2c1>>O=C(OCC#Cc1cnc2ccccc2c1)N(c1ccccc1)c1ccccc1
[NH4+].[Cl-].CC(C)([O-])C.[K+].N1=CC(=CC2=CC=CC=C12)C#CCO.C1(=CC=CC=C1)N(C(=O)Cl)C1=CC=CC=C1>>C1(=CC=CC=C1)N(C(=O)OCC#CC=1C=NC2=CC=CC=C2C1)C1=CC=CC=C1
Cl[C:2](=[O:1])[N:17]([c:18]1[cH:19][cH:20][cH:21][cH:22][cH:23]1)[c:24]1[cH:25][cH:26][cH:27][cH:28][cH:29]1.[OH:3][CH2:4][C:5]#[C:6][c:7]1[cH:8][n:9][c:10]2[cH:11][cH:12][cH:13][cH:14][c:15]2[cH:16]1>>[O:1]=[C:2]([O:3][CH2:4][C:5]#[C:6][c:7]1[cH:8][n:9][c:10]2[cH:11][cH:12][cH:13][cH:14][c:15]2[cH:16]1)[N:17]([c:18]1...
O=C(Cl)N(c1ccccc1)c1ccccc1.OCC#Cc1cnc2ccccc2c1
O=C(OCC#Cc1cnc2ccccc2c1)N(c1ccccc1)c1ccccc1
null
null
CC(C)(C)OC.C1CCOC1
Protection
Schotten-Baumann to ester
597fa7ba4ca169ec9e1d3b8730fbab27757ccde00143c31019a679c09b7b2b7f
562b6a5118cb63cbe5ff058f35135dc3f085de8b8ec7fa4ac4de518324eb826a
O=C(OCC#Cc1cnc2ccccc2c1)N(c1ccccc1)c1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#7:3](-[c:4])-[c:5].[#7;a:6]:[c:7]:[c:8]-[C:9]#[C:10]-[C:11]-[OH;D1;+0:12]>>[#7;a:6]:[c:7]:[c:8]-[C:9]#[C:10]-[C:11]-[O;H0;D2;+0:12]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#7:3](-[c:4])-[c:5]
null
[]
0
CELSIUS
2
HOUR
To a dry three-necked round-bottom flask equipped with nitrogen inlet and overhead stirrer was charged 3-(3-quinolyl)-2-propyn-1-ol (5 g, 27 mmol) in THF (50 ml) and the solution was cooled to 0° C. Potassium t-butoxide (3.6 g, 32 mmol) was then added followed by diphenylcarbamoyl chloride (6.9 g, 29.7 mmol). The mixtu...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Tertiary amide.Primary alcohol
Carbamic ester
null
null
c1ccc2ncccc2c1.c1ccccc1.c1ccccc1
HCl
CC(C)(C)OC.C1CCOC1
0
2
O=C(Cl)N(c1ccccc1)c1ccccc1.OCC#Cc1cnc2ccccc2c1>CC(C)(C)OC.C1CCOC1>O=C(OCC#Cc1cnc2ccccc2c1)N(c1ccccc1)c1ccccc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-bbde859250e14d4b9eae21d11a8ee9d3
CC(C)N(C(=O)Cl)C(C)C.OCC#Cc1cnc2ccccc2c1>>CC(C)N(C(=O)OCC#Cc1cnc2ccccc2c1)C(C)C
C(C)(C)N(C(=O)Cl)C(C)C.N1=CC(=CC2=CC=CC=C12)C#CCO.N1=CC(=CC2=CC=CC=C12)C#CCO.[NH4+].[Cl-].CC(C)([O-])C.[K+]>>C(C)(C)N(C(=O)OCC#CC=1C=NC2=CC=CC=C2C1)C(C)C
Cl[C:5]([N:4]([CH:2]([CH3:1])[CH3:3])[CH:21]([CH3:22])[CH3:23])=[O:6].[OH:7][CH2:8][C:9]#[C:10][c:11]1[cH:12][n:13][c:14]2[cH:15][cH:16][cH:17][cH:18][c:19]2[cH:20]1>>[CH3:1][CH:2]([CH3:3])[N:4]([C:5](=[O:6])[O:7][CH2:8][C:9]#[C:10][c:11]1[cH:12][n:13][c:14]2[cH:15][cH:16][cH:17][cH:18][c:19]2[cH:20]1)[CH:21]([CH3:22])...
CC(C)N(C(=O)Cl)C(C)C.OCC#Cc1cnc2ccccc2c1
CC(C)N(C(=O)OCC#Cc1cnc2ccccc2c1)C(C)C
null
null
CC(C)(C)OC.C1CCOC1
Protection
Schotten-Baumann to ester
597fa7ba4ca169ec9e1d3b8730fbab27757ccde00143c31019a679c09b7b2b7f
562b6a5118cb63cbe5ff058f35135dc3f085de8b8ec7fa4ac4de518324eb826a
c1ccc2ncccc2c1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#7:3](-[C:4])-[C:5].[#7;a:6]:[c:7]:[c:8]-[C:9]#[C:10]-[C:11]-[OH;D1;+0:12]>>[#7;a:6]:[c:7]:[c:8]-[C:9]#[C:10]-[C:11]-[O;H0;D2;+0:12]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#7:3](-[C:4])-[C:5]
null
[]
0
CELSIUS
2
HOUR
To a dry three-necked round-bottom flask equipped with nitrogen inlet and overhead stirrer was charged 3-(3-quinolyl)-2-propyn-1-ol (2 g, 10.8 mmol) (Scheme 1, Compound (3)) in THF (20 ml) and the solution was cooled to 0° C. Potassium t-butoxide (1.34 g, 11.9 mmol) was then added followed by diisopropylcarbamoyl chlor...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Tertiary amide.Primary alcohol
Carbamic ester
null
null
c1ccc2ncccc2c1
HCl
CC(C)(C)OC.C1CCOC1
0
2
CC(C)N(C(=O)Cl)C(C)C.OCC#Cc1cnc2ccccc2c1>CC(C)(C)OC.C1CCOC1>CC(C)N(C(=O)OCC#Cc1cnc2ccccc2c1)C(C)C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b4216f66d9d54bd8abacf998327fe60b
CI.O=c1cc(C(F)(F)F)c2cc([N+](=O)[O-])ccc2[nH]1>>Cn1c(=O)cc(C(F)(F)F)c2cc([N+](=O)[O-])ccc21
[N+](=O)([O-])C=1C=C2C(=CC(NC2=CC1)=O)C(F)(F)F.[OH-].[K+].CI>>CN1C(C=C(C2=CC(=CC=C12)[N+](=O)[O-])C(F)(F)F)=O
I[CH3:1].[nH:2]1[c:3](=[O:4])[cH:5][c:6]([C:7]([F:8])([F:9])[F:10])[c:11]2[cH:12][c:13]([N+:14](=[O:15])[O-:16])[cH:17][cH:18][c:19]12>>[CH3:1][n:2]1[c:3](=[O:4])[cH:5][c:6]([C:7]([F:8])([F:9])[F:10])[c:11]2[cH:12][c:13]([N+:14](=[O:15])[O-:16])[cH:17][cH:18][c:19]12
CI.O=c1cc(C(F)(F)F)c2cc([N+](=O)[O-])ccc2[nH]1
Cn1c(=O)cc(C(F)(F)F)c2cc([N+](=O)[O-])ccc21
null
null
null
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
8b34fe134eb750cc9638be1186f4b7fb81aa2af5327ea2fbd8cdd88c39c64638
7a358c636daddc97c1fb4c29f378044d7eac3f01815d9966e599841f642d631a
O=c1ccc2ccccc2[nH]1
I-[CH3;D1;+0:1].[O;D1;H0:2]=[c:3](:[c:4]):[nH;D2;+0:5]:[c:6](:[c:7]):[c:8]>>[CH3;D1;+0:1]-[n;H0;D3;+0:5](:[c:6](:[c:7]):[c:8]):[c:3](=[O;D1;H0:2]):[c:4]
57.6
[{"value": 57.0, "product": "CN1C(C=C(C2=CC(=CC=C12)[N+](=O)[O-])C(F)(F)F)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 57.6, "product": "CN1C(C=C(C2=CC(=CC=C12)[N+](=O)[O-])C(F)(F)F)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
6-Nitro-4-trifluoromethyl-1H-quinolin-2-one (2.50 g, 9.7 mmol) was methylated with KOH (5.46 g, 97.3 mmol) & MeI (6.1 mL, 97.3 mmol), as to give 1-methyl-6-nitro-4-trifluoromethyl-1H-quinolin-2-one (1.52 g, 57%): δH (CDCl3)=3.80 (s, 3H), 7.20 (s, 1H), 7.55 (d, 1H), 8.50 (dd, 1H), 8.75 (d, 1H). An EtOAc (50 mL) solution...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ccc2ncccc2c1
c1ccc2ncccc2c1
c1ccc2ncccc2c1
HI
null
null
null
CI.O=c1cc(C(F)(F)F)c2cc([N+](=O)[O-])ccc2[nH]1>>Cn1c(=O)cc(C(F)(F)F)c2cc([N+](=O)[O-])ccc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b782ccaa18914a638b92100784315792
Cn1c(=O)cc(C(F)(F)F)c2cc(N)ccc21.O=C=Nc1ccccc1>>Cn1c(=O)cc(C(F)(F)F)c2cc(NC(=O)Nc3ccccc3)ccc21
NC=1C=C2C(=CC(N(C2=CC1)C)=O)C(F)(F)F.C1(=CC=CC=C1)N=C=O.N1=CC=CC=C1>>CN1C(C=C(C2=CC(=CC=C12)NC(=O)NC1=CC=CC=C1)C(F)(F)F)=O
[CH3:1][n:2]1[c:3](=[O:4])[cH:5][c:6]([C:7]([F:8])([F:9])[F:10])[c:11]2[cH:12][c:13]([NH2:14])[cH:24][cH:25][c:26]12.[C:15](=[O:16])=[N:17][c:18]1[cH:19][cH:20][cH:21][cH:22][cH:23]1>>[CH3:1][n:2]1[c:3](=[O:4])[cH:5][c:6]([C:7]([F:8])([F:9])[F:10])[c:11]2[cH:12][c:13]([NH:14][C:15](=[O:16])[NH:17][c:18]3[cH:19][cH:20][...
Cn1c(=O)cc(C(F)(F)F)c2cc(N)ccc21.O=C=Nc1ccccc1
Cn1c(=O)cc(C(F)(F)F)c2cc(NC(=O)Nc3ccccc3)ccc21
null
null
CN(C)C=O
Acylation
Urea synthesis via isocyanate and primary amine
d39cd7dc52a79bb265ff8ef61ef7bf9dc7f7b5fb0150fcb4881bdfb18ab9c380
a5dc801930c765d2a435a0a2973e50163c305ba8e7641d6adbcc1550b7b96de7
O=C(Nc1ccccc1)Nc1ccc2[nH]c(=O)ccc2c1
[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4].[O;D1;H0:5]=[C;H0;D2;+0:6]=[N;H0;D2;+0:7]-[c:8](:[c:9]):[c:10]>>[O;D1;H0:5]=[C;H0;D3;+0:6](-[NH;D2;+0:1]-[c:2](:[c:3]):[c:4])-[NH;D2;+0:7]-[c:8](:[c:9]):[c:10]
80.3
[{"value": 80.0, "product": "CN1C(C=C(C2=CC(=CC=C12)NC(=O)NC1=CC=CC=C1)C(F)(F)F)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 80.3, "product": "CN1C(C=C(C2=CC(=CC=C12)NC(=O)NC1=CC=CC=C1)C(F)(F)F)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
16
HOUR
A solution of 6-amino-1-methyl-4-trifluoromethyl-1H-quinolin-2-one (Preparation 1, 48 mg, 200 μmol) in anhydrous DMF (2 mL) was treated with PhNCO (33 μL, 300 μmol) & pyridine (16 μL, 20 μmol). The mixture was stirred for 16 h & then partitioned between EtOAc (30 mL) & H2O (20 mL). The organic layer was washed with H2O...
10.6084/m9.figshare.5104873.v1
null
Isocyanate.Primary amine
Urea
null
null
c1ccc2ncccc2c1.c1ccccc1
null
CN(C)C=O
null
16
Cn1c(=O)cc(C(F)(F)F)c2cc(N)ccc21.O=C=Nc1ccccc1>CN(C)C=O>Cn1c(=O)cc(C(F)(F)F)c2cc(NC(=O)Nc3ccccc3)ccc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5fba2f7f0da44f38995cecb0aa6fbeb1
Cc1ccc(CCN=C=S)cc1.Cn1c(=O)cc(C(F)(F)F)c2cc(N)ccc21>>Cc1ccc(CCNC(=S)Nc2ccc3c(c2)c(C(F)(F)F)cc(=O)n3C)cc1
N1=CC=CC=C1.CC1=CC=C(CCN=C=S)C=C1.NC=1C=C2C(=CC(N(C2=CC1)C)=O)C(F)(F)F>>CN1C(C=C(C2=CC(=CC=C12)NC(=S)NCCC1=CC=C(C=C1)C)C(F)(F)F)=O
[CH3:1][c:2]1[cH:3][cH:4][c:5]([CH2:6][CH2:7][N:8]=[C:9]=[S:10])[cH:28][cH:29]1.[NH2:11][c:12]1[cH:13][cH:14][c:15]2[c:16]([cH:17]1)[c:18]([C:19]([F:20])([F:21])[F:22])[cH:23][c:24](=[O:25])[n:26]2[CH3:27]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([CH2:6][CH2:7][NH:8][C:9](=[S:10])[NH:11][c:12]2[cH:13][cH:14][c:15]3[c:16]([cH:17...
Cc1ccc(CCN=C=S)cc1.Cn1c(=O)cc(C(F)(F)F)c2cc(N)ccc21
Cc1ccc(CCNC(=S)Nc2ccc3c(c2)c(C(F)(F)F)cc(=O)n3C)cc1
null
null
CN1CCCC1=O
Heteroatom Alkylation and Arylation
thiourea
9037f368cdf8e91fcd9f93f4d9cf27991f85fa921c9d19c7875d3a77561f439b
0fbf3d6c8cd704ac451c2cf111f32090de5e76a9d41cce326e212c758f4ed46f
O=c1ccc2cc(NC(=S)NCCc3ccccc3)ccc2[nH]1
[C:1]-[C:2]-[N;H0;D2;+0:3]=[C;H0;D2;+0:4]=[S;D1;H0:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[C:1]-[C:2]-[NH;D2;+0:3]-[C;H0;D3;+0:4](=[S;D1;H0:5])-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]
20
[{"value": 20.0, "product": "CN1C(C=C(C2=CC(=CC=C12)NC(=S)NCCC1=CC=C(C=C1)C)C(F)(F)F)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
7
DAY
6-Amino-1-methyl-4-trifluoromethyl-1H-quinolin-2-one (Preparation 1, 200 μL of a 0.2 M solution in NMP, 40 μmol) was treated with pyridine (20 μL of a 0.2 M solution in NMP, 4 μmol) & 4-methylphenethyl isothiocyanate (240 μL of a 0.2 M solution in NMP, 48 μmol). After 7 d, the mixture was concentrated, then the residue...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Isothiocyanate
Thiourea
null
null
c1ccccc1.c1ccc2ncccc2c1
null
CN1CCCC1=O
null
168
Cc1ccc(CCN=C=S)cc1.Cn1c(=O)cc(C(F)(F)F)c2cc(N)ccc21>CN1CCCC1=O>Cc1ccc(CCNC(=S)Nc2ccc3c(c2)c(C(F)(F)F)cc(=O)n3C)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-1fa46e21f870488d806783ecc0222d0f
Cn1c(=O)cc(C(F)(F)F)c2cc(N)ccc21.S=C=NCCc1ccc(Cl)cc1>>Cn1c(=O)cc(C(F)(F)F)c2cc(NC(=S)NCCc3ccc(Cl)cc3)ccc21
NC=1C=C2C(=CC(N(C2=CC1)C)=O)C(F)(F)F.ClC1=CC=C(C=C1)CCN=C=S>>ClC1=CC=C(C=C1)CCNC(=S)NC=1C=C2C(=CC(N(C2=CC1)C)=O)C(F)(F)F
[CH3:1][n:2]1[c:3](=[O:4])[cH:5][c:6]([C:7]([F:8])([F:9])[F:10])[c:11]2[cH:12][c:13]([NH2:14])[cH:27][cH:28][c:29]12.[C:15](=[S:16])=[N:17][CH2:18][CH2:19][c:20]1[cH:21][cH:22][c:23]([Cl:24])[cH:25][cH:26]1>>[CH3:1][n:2]1[c:3](=[O:4])[cH:5][c:6]([C:7]([F:8])([F:9])[F:10])[c:11]2[cH:12][c:13]([NH:14][C:15](=[S:16])[NH:1...
Cn1c(=O)cc(C(F)(F)F)c2cc(N)ccc21.S=C=NCCc1ccc(Cl)cc1
Cn1c(=O)cc(C(F)(F)F)c2cc(NC(=S)NCCc3ccc(Cl)cc3)ccc21
null
null
CN1CCCC1=O
Heteroatom Alkylation and Arylation
thiourea
9037f368cdf8e91fcd9f93f4d9cf27991f85fa921c9d19c7875d3a77561f439b
0fbf3d6c8cd704ac451c2cf111f32090de5e76a9d41cce326e212c758f4ed46f
O=c1ccc2cc(NC(=S)NCCc3ccccc3)ccc2[nH]1
[C:1]-[C:2]-[N;H0;D2;+0:3]=[C;H0;D2;+0:4]=[S;D1;H0:5].[NH2;D1;+0:6]-[c:7](:[c:8]):[c:9]>>[C:1]-[C:2]-[NH;D2;+0:3]-[C;H0;D3;+0:4](=[S;D1;H0:5])-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]
40
[{"value": 40.0, "product": "ClC1=CC=C(C=C1)CCNC(=S)NC=1C=C2C(=CC(N(C2=CC1)C)=O)C(F)(F)F", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
Reaction of 6-amino-1-methyl-4-trifluoromethyl-1H-quinolin-2-one (Preparation 1, 200 μL of a 0.2 M solution in NMP, 40 μmol) with 2-(4-chlorophenyl)ethyl isothiocyanate (240 μL of a 0.2 M solution in NMP, 48 μmol), by the procedure outlined for Example 492, furnished the title compound (7.1 mg, 40%): RT=1.95 min; m/z (...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Isothiocyanate
Thiourea
null
null
c1ccc2ncccc2c1.c1ccccc1
null
CN1CCCC1=O
null
null
Cn1c(=O)cc(C(F)(F)F)c2cc(N)ccc21.S=C=NCCc1ccc(Cl)cc1>CN1CCCC1=O>Cn1c(=O)cc(C(F)(F)F)c2cc(NC(=S)NCCc3ccc(Cl)cc3)ccc21
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-70ccfe0370df4d57ac11e4966ad1c4e0
Nc1nc2ccc([N+](=O)[O-])cc2s1>>Nc1ccc2nc(N)sc2c1
NC=1SC2=C(N1)C=CC(=C2)[N+](=O)[O-].[H][H]>>NC=1SC2=C(N1)C=CC(=C2)N
O=[N+:1]([O-])[c:2]1[cH:3][cH:4][c:5]2[n:6][c:7]([NH2:8])[s:9][c:10]2[cH:11]1>>[NH2:1][c:2]1[cH:3][cH:4][c:5]2[n:6][c:7]([NH2:8])[s:9][c:10]2[cH:11]1
Nc1nc2ccc([N+](=O)[O-])cc2s1
Nc1ccc2nc(N)sc2c1
null
[Pd]
CO
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc2scnc2c1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]:[c:5]:[#16;a:6]>>[#16;a:6]:[c:5]:[c:4]:[c:2](-[NH2;D1;+0:1]):[c:3]
99.3
[{"value": 99.0, "product": "NC=1SC2=C(N1)C=CC(=C2)N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 99.3, "product": "NC=1SC2=C(N1)C=CC(=C2)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
2-Amino-6-nitrobenzothiazole (500 mg, 2.56 mmol) was dissolved in methanol (20 mL) and 10% palladium on carbon (50 mg) was added as a slurry in methanol (1 mL). The atmosphere was replaced with hydrogen and the suspension was stirred overnight. The catalyst was removed by suction filtration and the solvent evaporated t...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccc2scnc2c1
Other
[Pd].CO
null
8
Nc1nc2ccc([N+](=O)[O-])cc2s1>[Pd].CO>Nc1ccc2nc(N)sc2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-951fd2859fd144deb086a5a97529b901
Nc1ccc2c(c1)CCC2.O=CO>>O=CNc1ccc2c(c1)CCC2
NC=1C=C2CCCC2=CC1.C(=O)O.Cl.CN(CCCN=C=NCC)C.C(C)(C)N(CC)C(C)C>>C(=O)NC=1C=C2CCCC2=CC1
[NH2:3][c:4]1[cH:5][cH:6][c:7]2[c:8]([cH:9]1)[CH2:10][CH2:11][CH2:12]2.O[CH:2]=[O:1]>>[O:1]=[CH:2][NH:3][c:4]1[cH:5][cH:6][c:7]2[c:8]([cH:9]1)[CH2:10][CH2:11][CH2:12]2
Nc1ccc2c(c1)CCC2.O=CO
O=CNc1ccc2c(c1)CCC2
null
null
CN(C)C=O
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
c1ccc2c(c1)CCC2
O-[CH;D2;+0:1]=[O;D1;H0:2].[NH2;D1;+0:3]-[c:4](:[c:5]):[c:6]>>[O;D1;H0:2]=[CH;D2;+0:1]-[NH;D2;+0:3]-[c:4](:[c:5]):[c:6]
93.3
[{"value": 93.0, "product": "C(=O)NC=1C=C2CCCC2=CC1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 93.3, "product": "C(=O)NC=1C=C2CCCC2=CC1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To a solution of 5-aminoindane (7.53 g, 56.5 mmol) in DMF (100 mL) was added formic acid (2.2 mL, 58.3 mmol), 1-(3-dimethylaminopropyl)-3-ethylcarbodiimide hydrochloride (10.94 g, 57 mmol) and diisopropylethylamine (19.7 mL, 0.11 mol). The resulting solution was stirred overnight and then partitioned between saturated ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccc2c(c1)CCC2
HO-
CN(C)C=O
null
8
Nc1ccc2c(c1)CCC2.O=CO>CN(C)C=O>O=CNc1ccc2c(c1)CCC2
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a7aab29217ca490d8d969149d8fdcd45
CCOC(=O)C(=NO)C(=O)CCl.NC(=S)c1ccccc1>>CCOC(=O)C(=NO)c1csc(-c2ccccc2)n1
ClCC(C(C(=O)OCC)=NO)=O.C(C1=CC=CC=C1)(=S)N>>N(O)=C(C(=O)OCC)C=1N=C(SC1)C1=CC=CC=C1
O=[C:9]([C:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])=[N:7][OH:8])[CH2:10]Cl.[S:11]=[C:12]([c:13]1[cH:14][cH:15][cH:16][cH:17][cH:18]1)[NH2:19]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[C:6](=[N:7][OH:8])[c:9]1[cH:10][s:11][c:12](-[c:13]2[cH:14][cH:15][cH:16][cH:17][cH:18]2)[n:19]1
CCOC(=O)C(=NO)C(=O)CCl.NC(=S)c1ccccc1
CCOC(=O)C(=NO)c1csc(-c2ccccc2)n1
null
null
C1=CC=CC=C1
Aromatic Heterocycle Formation
OtherReaction
21eb8c7cda3c7fc14309a0c556334226f1a9147c334386d33bc70341830a82ec
9f145257a80f08f1a7a6ee36c84cd4115965bd63128f36de61c7ed688ad2603c
c1ccc(-c2nccs2)cc1
Cl-[CH2;D2;+0:1]-[C;H0;D3;+0:2](=O)-[C:3](=[#7:4]-[O;D1;H1:5])-[C:6](=[O;D1;H0:7])-[#8:8]-[C:9].[NH2;D1;+0:10]-[C;H0;D3;+0:11](=[S;H0;D1;+0:12])-[c;H0;D3;+0:13](:[c:14]:[c:15]):[c:16]:[c:17]>>[C:9]-[#8:8]-[C:6](=[O;D1;H0:7])-[C:3](=[#7:4]-[O;D1;H1:5])-[c;H0;D3;+0:2]1:[cH;D2;+0:1]:[s;H0;D2;+0:12]:[c;H0;D3;+0:11](-[c;H0;...
107.9
[{"value": 107.9, "product": "N(O)=C(C(=O)OCC)C=1N=C(SC1)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
A solution of ethyl γ-chloro-α-oximinoacetoacetate (2.10 g, 10.8 mmol) and thiobenzamide (1.49 g, 10.8 mmol) in dry benzene (15 mL) was heated to reflux. After 4 hours, the reaction mixture was poured onto NaHCO3 (sat., aq., 50 mL); The resulting mixture was extracted with ethyl acetate (2×50 mL); and the combined extr...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ketone.Thioamide
null
null
c1cscn1
c1cscn1.c1ccccc1
HCl
C1=CC=CC=C1
null
4
CCOC(=O)C(=NO)C(=O)CCl.NC(=S)c1ccccc1>C1=CC=CC=C1>CCOC(=O)C(=NO)c1csc(-c2ccccc2)n1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-b719000289c949c1b73f29564e672469
CO.Nc1ccc(C(=O)O)cn1>>COC(=O)c1ccc(N)nc1
NC1=NC=C(C(=O)O)C=C1.S(O)(O)(=O)=O.CO>>NC1=NC=C(C(=O)OC)C=C1
[CH3:1][OH:2].O[C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([NH2:9])[n:10][cH:11]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([NH2:9])[n:10][cH:11]1
CO.Nc1ccc(C(=O)O)cn1
COC(=O)c1ccc(N)nc1
null
null
null
Protection
Esterification of Carboxylic Acids
9cecdbd189c6f9c3648521d17154d013842a5498de4e76e65efb1d842973340b
af0b8064f2e82ebe66c4c29d2391785ac1b993104265ccdc4d67ca79e36fa3c8
c1ccncc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]:[#7;a:6]:[c:7].[C;D1;H3:8]-[OH;D1;+0:9]>>[C;D1;H3:8]-[O;H0;D2;+0:9]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]:[#7;a:6]:[c:7]
30
[{"value": 30.0, "product": "NC1=NC=C(C(=O)OC)C=C1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A suspension of 6-aminonicotinic acid (2.0 g, 14.5 mmol) and sulfuric acid (2 mL) in methanol (125 mL) was heated at reflux overnight. The solution was cooled, the methanol evaporated and the residue was taken up in water (100 mL) and made basic with NaHCO3 (s), causing a white solid to precipitate. The mixture was ext...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Methanol
Ester
null
null
c1ccncc1
HO-
null
null
null
CO.Nc1ccc(C(=O)O)cn1>>COC(=O)c1ccc(N)nc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-5df7c6a4559e4c7fadd29da15281fbc1
O=C(O)c1cccnc1Cl>>COC(=O)c1cccnc1Cl
C(=O)(O)[O-].[Na+].ClC1=C(C(=O)O)C=CC=N1.S(O)(O)(=O)=O.O>>ClC1=C(C(=O)OC)C=CC=N1
[OH:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][cH:8][n:9][c:10]1[Cl:11]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][cH:8][n:9][c:10]1[Cl:11]
O=C(O)c1cccnc1Cl
COC(=O)c1cccnc1Cl
null
null
CO
Miscellaneous
Protection of carboxylic acid
56520e0abb4535dce9a663824ca803b71c2c0dd72dfd246317d953596a987bd2
2ccc7a30191c2c171b49e8a0217bee87430687dd0f567141eca025a75b7e3136
c1ccncc1
[#7;a:1]:[c:2]:[c:3]-[C:4](=[O;D1;H0:5])-[OH;D1;+0:6]>>[#7;a:1]:[c:2]:[c:3]-[C:4](=[O;D1;H0:5])-[O;H0;D2;+0:6]-[C;D1;H3:7]
40
[{"value": 40.0, "product": "ClC1=C(C(=O)OC)C=CC=N1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 2-chloronicotinic acid (1.61 g, 10.2 mmol) and sulfuric acid (0.5 mL) in methanol (30 mL) was stirred at reflux overnight. The solution was poured into water (100 mL) and neutralised with NaHCO3 (s) before being extracted with 1:1 hexane/ethyl acetate (3×40 mL). The solvents were dried (MgSO4) and evapora...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Ester
null
null
c1ccncc1
Other
CO
null
null
O=C(O)c1cccnc1Cl>CO>COC(=O)c1cccnc1Cl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-9b586bba5e9a41db8c92d9207fc46e12
CCC(N)=S.CCOC(=O)C(=NO)C(=O)CCl>>CCOC(=O)C(=NO)c1csc(CC)n1
ClCC(C(C(=O)OCC)=NO)=O.C(CC)(=S)N>>N(O)=C(C(=O)OCC)C=1N=C(SC1)CC
[S:11]=[C:12]([CH2:13][CH3:14])[NH2:15].O=[C:9]([C:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])=[N:7][OH:8])[CH2:10]Cl>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[C:6](=[N:7][OH:8])[c:9]1[cH:10][s:11][c:12]([CH2:13][CH3:14])[n:15]1
CCC(N)=S.CCOC(=O)C(=NO)C(=O)CCl
CCOC(=O)C(=NO)c1csc(CC)n1
null
null
C1=CC=CC=C1
Aromatic Heterocycle Formation
OtherReaction
21eb8c7cda3c7fc14309a0c556334226f1a9147c334386d33bc70341830a82ec
9f145257a80f08f1a7a6ee36c84cd4115965bd63128f36de61c7ed688ad2603c
c1cscn1
Cl-[CH2;D2;+0:1]-[C;H0;D3;+0:2](=O)-[C:3](=[#7:4]-[O;D1;H1:5])-[C:6](=[O;D1;H0:7])-[#8:8]-[C:9].[C;D1;H3:10]-[C:11]-[C;H0;D3;+0:12](-[NH2;D1;+0:13])=[S;H0;D1;+0:14]>>[C:9]-[#8:8]-[C:6](=[O;D1;H0:7])-[C:3](=[#7:4]-[O;D1;H1:5])-[c;H0;D3;+0:2]1:[cH;D2;+0:1]:[s;H0;D2;+0:14]:[c;H0;D3;+0:12](-[C:11]-[C;D1;H3:10]):[n;H0;D2;+0...
35.3
[{"value": 35.3, "product": "N(O)=C(C(=O)OCC)C=1N=C(SC1)CC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
A solution of ethyl γ-chloro-α-oximinoacetoacetate (2.00 g, 10.3 mmol) and thiopropionamide (0.92 g, 10.3 mmol) in dry benzene (15 mL) was heated to reflux. After 4 hours, the reaction mixture was poured onto NaHCO3 (sat. aq., 50 mL), The resulting mixture was extracted with ethyl acetate (2×50 mL), and the combined ex...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ketone.Thioamide
null
null
c1cscn1
c1cscn1
HCl
C1=CC=CC=C1
null
4
CCC(N)=S.CCOC(=O)C(=NO)C(=O)CCl>C1=CC=CC=C1>CCOC(=O)C(=NO)c1csc(CC)n1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4908647c9fd043d7b326254adfe97735
CCC(N)=S.CCOC(=O)C(=NO)C(=O)CCl>>CCOC(=O)C(=NO)c1csc(CC)n1
ClCC(C(C(=O)OCC)=NO)=O.C(CC)(=S)N>>N(O)=C(C(=O)OCC)C=1N=C(SC1)CC
[S:11]=[C:12]([CH2:13][CH3:14])[NH2:15].O=[C:9]([C:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])=[N:7][OH:8])[CH2:10]Cl>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[C:6](=[N:7][OH:8])[c:9]1[cH:10][s:11][c:12]([CH2:13][CH3:14])[n:15]1
CCC(N)=S.CCOC(=O)C(=NO)C(=O)CCl
CCOC(=O)C(=NO)c1csc(CC)n1
null
null
C1=CC=CC=C1
Aromatic Heterocycle Formation
OtherReaction
21eb8c7cda3c7fc14309a0c556334226f1a9147c334386d33bc70341830a82ec
9f145257a80f08f1a7a6ee36c84cd4115965bd63128f36de61c7ed688ad2603c
c1cscn1
Cl-[CH2;D2;+0:1]-[C;H0;D3;+0:2](=O)-[C:3](=[#7:4]-[O;D1;H1:5])-[C:6](=[O;D1;H0:7])-[#8:8]-[C:9].[C;D1;H3:10]-[C:11]-[C;H0;D3;+0:12](-[NH2;D1;+0:13])=[S;H0;D1;+0:14]>>[C:9]-[#8:8]-[C:6](=[O;D1;H0:7])-[C:3](=[#7:4]-[O;D1;H1:5])-[c;H0;D3;+0:2]1:[cH;D2;+0:1]:[s;H0;D2;+0:14]:[c;H0;D3;+0:12](-[C:11]-[C;D1;H3:10]):[n;H0;D2;+0...
35.3
[{"value": 35.3, "product": "N(O)=C(C(=O)OCC)C=1N=C(SC1)CC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of ethyl γ-chloro-α-oximinoacetoacetate (2.00 g, 10.3 mmol) and thiopropionamide (0.92 g, 10.3 mmol) in dry benzene (15 mL) was heated at reflux. After 4 hours the reaction mixture was poured onto NaHCO3 (sat. aq., 50 mL), The resulting mixture was extracted with ethyl acetate (2×50 mL), and the combined ext...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ketone.Thioamide
null
null
c1cscn1
c1cscn1
HCl
C1=CC=CC=C1
null
null
CCC(N)=S.CCOC(=O)C(=NO)C(=O)CCl>C1=CC=CC=C1>CCOC(=O)C(=NO)c1csc(CC)n1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f6398d85ae1e499096b7dc403b7c24e0
C=CC(=O)OCC(CC)CCCC>>CCCCC(CC)C(=O)O
C(C=C)(=O)OCC(CCCC)CC.C([O-])([O-])=O.[Cs+].[Cs+]>>CCCCC(CC)C(=O)O
C(C(C[O:10][C:8]([CH:5]=[CH2:6])=[O:9])[CH2:4][CH2:3][CH2:2][CH3:1])[CH3:7]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH:5]([CH2:6][CH3:7])[C:8](=[O:9])[OH:10]
C=CC(=O)OCC(CC)CCCC
CCCCC(CC)C(=O)O
null
null
C(C)#N
Miscellaneous
OtherReaction
7bb1c6a47ceff39dbfe124fd8262f8cabbf022e9f3f42a469d88b73802e7ca41
e688aeafd627b2d2fb9627b228ddfee0f20a7656c4b9b14ac8ece839b175abbe
null
[C:1]-[C:2]-[CH2;D2;+0:3]-C(-C-[CH3;D1;+0:4])-C-[O;H0;D2;+0:5]-[C:6](=[O;D1;H0:7])-[CH;D2;+0:8]=[CH2;D1;+0:9]>>[C:1]-[C:2]-[CH2;D2;+0:3]-[CH;D3;+0:8](-[CH2;D2;+0:9]-[CH3;D1;+0:4])-[C:6](=[O;D1;H0:7])-[OH;D1;+0:5]
399.2
[{"value": 88.0, "product": "CCCCC(CC)C(=O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 399.2, "product": "CCCCC(CC)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
24
HOUR
A mixture of TMIT (1.0 g, 6.33 mmol), 2-ethylhexyl acrylate (1.16 g, 6.33 mmol) and cesium carbonate (1.0 g, 3.3 mmol) in acetonitrile (15 mL) was stirred at room temperature for 24 h. The reaction mixture was filtered to separate solid cesium carbonate and solvent was evaporated from the filtrate to obtain the product...
10.6084/m9.figshare.5104873.v1
null
Ester.Vinyl
Carboxylic acid
null
null
null
Other
C(C)#N
null
24
C=CC(=O)OCC(CC)CCCC>C(C)#N>CCCCC(CC)C(=O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-e54e313d973542d5b345a9880f543028
C=CC(=O)OCC(CC)CCCC.CCCCC(CC)C(=O)O>>CC(=O)CC(C)C.CC(C)=O.CCC(C)=O.O=C1CCCCC1
CCCCC(CC)C(=O)O.C(C=C)(=O)OCC(CCCC)CC.C([O-])([O-])=O.[Cs+].[Cs+]>>CC(=O)C.C(C(C)C)C(=O)C.C(C)C(=O)C.C1(CCCCC1)=O
C([CH:2]([CH2:1]O[C:18](=[O:17])[CH:23]=[CH2:22])[CH2:4][CH2:5][CH2:6][CH3:8])[CH3:19].[O:3]=[C:15]([CH:14]([CH2:13][CH3:12])[CH2:20][CH2:21][CH2:7][CH3:10])[OH:16]>>[CH3:1][C:2](=[O:3])[CH2:4][CH:5]([CH3:6])[CH3:7].[CH3:8][C:9]([CH3:10])=[O:11].[CH3:12][CH2:13][C:14]([CH3:15])=[O:16].[O:17]=[C:18]1[CH2:19][CH2:20][CH2...
C=CC(=O)OCC(CC)CCCC.CCCCC(CC)C(=O)O
CC(=O)CC(C)C.CC(C)=O.CCC(C)=O.O=C1CCCCC1
null
null
C(C)#N
Functional Group Interconversion
OtherReaction
fd4745e6d70d8f0443751cecf30ddbdcc0bd81f584e0728f9c641d8772c5bad6
ca7529c6d5fb6e28032a33cd0c34ce7963c71f4e51fd214696a939d1402658f7
O=C1CCCCC1
[C;D1;H3:1]-[C:2]-[CH;D3;+0:3](-[CH2;D2;+0:4]-[CH2;D2;+0:5]-[CH2;D2;+0:6]-[CH3;D1;+0:7])-[C;H0;D3;+0:8](=[O;H0;D1;+0:9])-[OH;D1;+0:10].[CH2;D1;+0:11]=[CH;D2;+0:12]-[C;H0;D3;+0:13](=[O;D1;H0:14])-O-[CH2;D2;+0:15]-[CH;D3;+0:16](-C-[CH3;D1;+0:17])-[C:18]-[CH2;D2;+0:19]-[CH2;D2;+0:20]-[CH3;D1;+0:21]>>[C;D1;H3:1]-[C:2]-[C;H...
99
[{"value": 99.0, "product": "CC(=O)C.C(C(C)C)C(=O)C.C(C)C(=O)C.C1(CCCCC1)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A procedure similar to that of Example 2 was used for the reaction with 2-EHA. Starting from the TAIT product described in the preceding paragraph (1.0 g, ca. 4.5 mmol), 2-ethylhexyl acrylate (0.82 g, 4.5 mmol) and cesium carbonate (0.75 g, 2.25 mmol) in acetonitrile (20 mL), the product was isolated as a yellow oil an...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Ester.Vinyl
Ketone.Ketone.Ketone.Ketone
null
C1CCCCC1
C1CCCCC1
null
C(C)#N
null
null
C=CC(=O)OCC(CC)CCCC.CCCCC(CC)C(=O)O>C(C)#N>CC(=O)CC(C)C.CC(C)=O.CCC(C)=O.O=C1CCCCC1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-052671d368d5428ab7a7b87c87dd57b7
C=CC(=O)OCC(CC)CCCC>>CCCCC(CC)C(=O)O
C(C=C)(=O)OCC(CCCC)CC.C([O-])([O-])=O.[Cs+].[Cs+]>>CCCCC(CC)C(=O)O
C(C(C[O:10][C:8]([CH:5]=[CH2:6])=[O:9])[CH2:4][CH2:3][CH2:2][CH3:1])[CH3:7]>>[CH3:1][CH2:2][CH2:3][CH2:4][CH:5]([CH2:6][CH3:7])[C:8](=[O:9])[OH:10]
C=CC(=O)OCC(CC)CCCC
CCCCC(CC)C(=O)O
null
null
CCCCCC
Miscellaneous
OtherReaction
7bb1c6a47ceff39dbfe124fd8262f8cabbf022e9f3f42a469d88b73802e7ca41
e688aeafd627b2d2fb9627b228ddfee0f20a7656c4b9b14ac8ece839b175abbe
null
[C:1]-[C:2]-[CH2;D2;+0:3]-C(-C-[CH3;D1;+0:4])-C-[O;H0;D2;+0:5]-[C:6](=[O;D1;H0:7])-[CH;D2;+0:8]=[CH2;D1;+0:9]>>[C:1]-[C:2]-[CH2;D2;+0:3]-[CH;D3;+0:8](-[CH2;D2;+0:9]-[CH3;D1;+0:4])-[C:6](=[O;D1;H0:7])-[OH;D1;+0:5]
8,029.1
[{"value": 86.0, "product": "CCCCC(CC)C(=O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 8029.1, "product": "CCCCC(CC)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of TMIT (2.37 g, 15 mmol), 2-ethylhexyl acrylate (2.76 g, 15 mmol) and cesium carbonate (0.12 g, 0.38 mmol, 2.5 mole % based on acrylate) was heated in a sand bath at 100–120 ° C. for 2 h, while the progress of the reaction was being followed by IR spectroscopy. The reaction mixture was cooled to room tempera...
10.6084/m9.figshare.5104873.v1
null
Ester.Vinyl
Carboxylic acid
null
null
null
Other
CCCCCC
null
null
C=CC(=O)OCC(CC)CCCC>CCCCCC>CCCCC(CC)C(=O)O
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-dd257e48db34464b8c956bd6616382ef
CC(C)(C)OC(=O)OC(=O)OC(C)(C)C.CSc1ccc2cc(C)[nH]c2c1>>CSc1ccc2cc(C)n(C(=O)OC(C)(C)C)c2c1
CC=1NC2=CC(=CC=C2C1)SC.O(C(=O)OC(C)(C)C)C(=O)OC(C)(C)C>>C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)SC)C
CC(C)(C)OC(=O)O[C:11](=[O:12])[O:13][C:14]([CH3:15])([CH3:16])[CH3:17].[CH3:1][S:2][c:3]1[cH:4][cH:5][c:6]2[cH:7][c:8]([CH3:9])[nH:10][c:18]2[cH:19]1>>[CH3:1][S:2][c:3]1[cH:4][cH:5][c:6]2[cH:7][c:8]([CH3:9])[n:10]([C:11](=[O:12])[O:13][C:14]([CH3:15])([CH3:16])[CH3:17])[c:18]2[cH:19]1
CC(C)(C)OC(=O)OC(=O)OC(C)(C)C.CSc1ccc2cc(C)[nH]c2c1
CSc1ccc2cc(C)n(C(=O)OC(C)(C)C)c2c1
null
CN(C)C=1C=CN=CC1
CC#N
Acylation
Boc amine protection with Boc anhydride
59b538532b052ee63d6e8c6fd2ceac74caf9447c270a35d5982b50412a6732f0
ba6477f131c4ae5c5d3bddeb26f4fd18d7127f5da39407a22603c0ae12b886c7
c1ccc2[nH]ccc2c1
C-C(-C)(-C)-O-C(=O)-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C:4](-[C;D1;H3:5])(-[C;D1;H3:6])-[C;D1;H3:7].[C;D1;H3:8]-[c:9]1:[c:10]:[c:11]:[c:12](:[c:13]):[nH;D2;+0:14]:1>>[C;D1;H3:5]-[C:4](-[C;D1;H3:6])(-[C;D1;H3:7])-[#8:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[n;H0;D3;+0:14]1:[c:12](:[c:13]):[c:11]:[c:10]:[c:9]:1-[C;D1;H3:8]
null
[]
null
null
null
null
2-Methyl-6-methylthioindole (13.9 g) prepared according to Allais A. et al. Eur. J. Med. Chem.—Chim. Ther. (1975), 10(2), 187–99, was dissolved in CH3CN (150 mL) followed by the addition of (BOC)2O (18 g) with 480 mg DMAP. After 5 h the mixture was evaporated to dryness and the resulting 2-methyl-6-methylsulfanyl-indol...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Carbonic Ester.Carbonic Ester.Boc.Boc
Ether.Boc
c1ccc2[nH]ccc2c1
c1ccc2cc[nH]c2c1
c1ccc2cc[nH]c2c1
HO-
CN(C)C=1C=CN=CC1.CC#N
null
null
CC(C)(C)OC(=O)OC(=O)OC(C)(C)C.CSc1ccc2cc(C)[nH]c2c1>CN(C)C=1C=CN=CC1.CC#N>CSc1ccc2cc(C)n(C(=O)OC(C)(C)C)c2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d3e61d42c900447d958fe32e9fec35c7
CSc1ccc2cc(C)n(C(=O)OC(C)(C)C)c2c1>>Cc1cc2ccc(S(C)(=O)=O)cc2n1C(=O)OC(C)(C)C
C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)SC)C.OOS(=O)[O-].[K+].CO.O>>C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)S(=O)(=O)C)C
[CH3:1][c:2]1[cH:3][c:4]2[cH:5][cH:6][c:7]([S:8][CH3:9])[cH:12][c:13]2[n:14]1[C:15](=[O:16])[O:17][C:18]([CH3:19])([CH3:20])[CH3:21]>>[CH3:1][c:2]1[cH:3][c:4]2[cH:5][cH:6][c:7]([S:8]([CH3:9])(=[O:10])=[O:11])[cH:12][c:13]2[n:14]1[C:15](=[O:16])[O:17][C:18]([CH3:19])([CH3:20])[CH3:21]
CSc1ccc2cc(C)n(C(=O)OC(C)(C)C)c2c1
Cc1cc2ccc(S(C)(=O)=O)cc2n1C(=O)OC(C)(C)C
null
null
null
Oxidation
OtherReaction
20dd6d48007b4fe7cd760226f21413eb5e71e6468db112596c2e7ea4858c8ac1
5cedc1bf0f43f21d78a249521ecfcec19fc5ac4895c41eed0e84f0c2618149fa
c1ccc2[nH]ccc2c1
[#7;a:1]:[c:2]:[c:3]:[c:4](-[S;H0;D2;+0:5]-[C;D1;H3:6]):[c:7]>>[#7;a:1]:[c:2]:[c:3]:[c:4](-[S;H0;D4;+0:5](-[C;D1;H3:6])(=[O;D1;H0:8])=[O;D1;H0:9]):[c:7]
null
[]
null
null
null
null
The product of step 1 (20.3 g) was treated with 135 g OXONE™ in 300 mL 1:1 MeOH/water for 2 h. The mixture was partitioned between methylene chloride and water, the organic layer was separated, washed, dried, and evaporated to dryness to yield 6-methanesulfonyl-2-methyl-indole-1-carboxylic acid tert-butyl ester (16 g) ...
10.6084/m9.figshare.5104873.v1
null
Monosulfide
Sulfone
null
null
c1ccc2cc[nH]c2c1
null
null
null
null
CSc1ccc2cc(C)n(C(=O)OC(C)(C)C)c2c1>>Cc1cc2ccc(S(C)(=O)=O)cc2n1C(=O)OC(C)(C)C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-a767b45ee400491aa014c4ceb48dbe06
Cc1cc2ccc(S(C)(=O)=O)cc2n1C(=O)OC(C)(C)C>>Cc1cc2ccc(S(C)(=O)=O)cc2[nH]1
C(C)(C)(C)OC(=O)N1C(=CC2=CC=C(C=C12)S(=O)(=O)C)C.C(=O)(C(F)(F)F)O>>CS(=O)(=O)C1=CC=C2C=C(NC2=C1)C
CC(C)(C)OC(=O)[n:14]1[c:2]([CH3:1])[cH:3][c:4]2[cH:5][cH:6][c:7]([S:8]([CH3:9])(=[O:10])=[O:11])[cH:12][c:13]21>>[CH3:1][c:2]1[cH:3][c:4]2[cH:5][cH:6][c:7]([S:8]([CH3:9])(=[O:10])=[O:11])[cH:12][c:13]2[nH:14]1
Cc1cc2ccc(S(C)(=O)=O)cc2n1C(=O)OC(C)(C)C
Cc1cc2ccc(S(C)(=O)=O)cc2[nH]1
null
null
C(Cl)Cl
Reduction
Boc amine deprotection
3ccb08daaf21d271cf107ee1f39fc83392e4e5d2cdab9bb060bd71daac89b2f3
e1bf5a54b1f87284564f107662531aec2aff7de801e4606340967b38924afb28
c1ccc2[nH]ccc2c1
C-C(-C)(-C)-O-C(=O)-[n;H0;D3;+0:1]1:[c:2](:[c:3]):[c:4]:[c:5]:[c:6]:1-[C;D1;H3:7]>>[C;D1;H3:7]-[c:6]1:[c:5]:[c:4]:[c:2](:[c:3]):[nH;D2;+0:1]:1
null
[]
null
null
8
HOUR
The above product of step 2 was dissolved in 100 mL methylene chloride and treated with 12 mL TFA. After stirring overnight, the volatiles were removed and the product crystallized from 10:1 methylene chloride/MeOH. In this way 8.0 g of 6-methanesulfonyl-2-methyl-1H-indole was obtained. Conditions: See reaction.notes.p...
10.6084/m9.figshare.5104873.v1
null
Ether.Boc
null
c1ccc2cc[nH]c2c1
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
HO-
C(Cl)Cl
null
8
Cc1cc2ccc(S(C)(=O)=O)cc2n1C(=O)OC(C)(C)C>C(Cl)Cl>Cc1cc2ccc(S(C)(=O)=O)cc2[nH]1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-528a8c9dd1f74cc2a0a17ba4243f5107
Cc1cc2ccc(S(C)(=O)=O)cc2[nH]1.Fc1ccc(S)cc1>>Cc1[nH]c2cc(S(C)(=O)=O)ccc2c1Sc1ccc(F)cc1
C1=CC=C(C=C1)I(OC(=O)C(F)(F)F)OC(=O)C(F)(F)F.CS(=O)(=O)C1=CC=C2C=C(NC2=C1)C.FC1=CC=C(C=C1)S>>FC1=CC=C(C=C1)SC1=C(NC2=CC(=CC=C12)S(=O)(=O)C)C
[CH3:1][c:2]1[nH:3][c:4]2[cH:5][c:6]([S:7]([CH3:8])(=[O:9])=[O:10])[cH:11][cH:12][c:13]2[cH:14]1.[SH:15][c:16]1[cH:17][cH:18][c:19]([F:20])[cH:21][cH:22]1>>[CH3:1][c:2]1[nH:3][c:4]2[cH:5][c:6]([S:7]([CH3:8])(=[O:9])=[O:10])[cH:11][cH:12][c:13]2[c:14]1[S:15][c:16]1[cH:17][cH:18][c:19]([F:20])[cH:21][cH:22]1
Cc1cc2ccc(S(C)(=O)=O)cc2[nH]1.Fc1ccc(S)cc1
Cc1[nH]c2cc(S(C)(=O)=O)ccc2c1Sc1ccc(F)cc1
null
null
FC(C(C(F)(F)F)O)(F)F
Heteroatom Alkylation and Arylation
OtherReaction
6d0ae58eb1269904d7dda169c1c9a22d9d8065e25d20aca85acf2d11bcd1657c
a20e50d7df818b91ffc2e826d304ad74f6246978a284c599e867e2d806b7437e
c1ccc(Sc2c[nH]c3ccccc23)cc1
[C;D1;H3:1]-[c:2]1:[#7;a:3]:[c:4](:[c:5]):[c:6](:[c:7]):[cH;D2;+0:8]:1.[SH;D1;+0:9]-[c:10](:[c:11]):[c:12]>>[C;D1;H3:1]-[c:2]1:[#7;a:3]:[c:4](:[c:5]):[c:6](:[c:7]):[c;H0;D3;+0:8]:1-[S;H0;D2;+0:9]-[c:10](:[c:11]):[c:12]
43.2
[{"value": 43.2, "product": "FC1=CC=C(C=C1)SC1=C(NC2=CC(=CC=C12)S(=O)(=O)C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
A solution of 6-methanesulfonyl-2-methyl-1H-indole (207 mg, 1 mmol) in 6 mL of hexafluoroisopropanol was treated with 4-fluorothiophenol (2 mmol) followed by addition of PIFA (1.5 mmol). The dark colored solution was stirred for 30 minutes followed by partitioning between EtOAc and water. Purification by TLC (2:1 hexan...
10.6084/m9.figshare.5104873.v1
null
Aromatic thiol
Monosulfide
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.c1ccccc1
null
FC(C(C(F)(F)F)O)(F)F
null
0.5
Cc1cc2ccc(S(C)(=O)=O)cc2[nH]1.Fc1ccc(S)cc1>FC(C(C(F)(F)F)O)(F)F>Cc1[nH]c2cc(S(C)(=O)=O)ccc2c1Sc1ccc(F)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-75e9fdcbd15d450b90e60bf40947cf41
Cc1cc2ccc(S(C)(=O)=O)cc2[nH]1.O=Cc1ccc(Br)cc1>>Cc1[nH]c2cc(S(C)(=O)=O)ccc2c1Cc1ccc(Br)cc1
[SiH](CC)(CC)CC.CS(=O)(=O)C1=CC=C2C=C(NC2=C1)C.BrC1=CC=C(C=O)C=C1.[Si](C)(C)(C)OS(=O)(=O)C(F)(F)F>>BrC1=CC=C(CC2=C(NC3=CC(=CC=C23)S(=O)(=O)C)C)C=C1
[CH3:1][c:2]1[nH:3][c:4]2[cH:5][c:6]([S:7]([CH3:8])(=[O:9])=[O:10])[cH:11][cH:12][c:13]2[cH:14]1.O=[CH:15][c:16]1[cH:17][cH:18][c:19]([Br:20])[cH:21][cH:22]1>>[CH3:1][c:2]1[nH:3][c:4]2[cH:5][c:6]([S:7]([CH3:8])(=[O:9])=[O:10])[cH:11][cH:12][c:13]2[c:14]1[CH2:15][c:16]1[cH:17][cH:18][c:19]([Br:20])[cH:21][cH:22]1
Cc1cc2ccc(S(C)(=O)=O)cc2[nH]1.O=Cc1ccc(Br)cc1
Cc1[nH]c2cc(S(C)(=O)=O)ccc2c1Cc1ccc(Br)cc1
null
null
C(Cl)Cl
C-C Coupling
OtherReaction
6f6cce4aab73ee59c23ac064427a037ebc27409d1dc32dbc2e0b3f5346069911
cedc9d4b791e43eacf8e7ecfa6a98d1dc0438794e96e4f1c4bef436b78f82bd8
c1ccc(Cc2c[nH]c3ccccc23)cc1
O=[CH;D2;+0:1]-[c:2](:[c:3]):[c:4].[C;D1;H3:5]-[c:6]1:[#7;a:7]:[c:8](:[c:9]):[c:10](:[c:11]):[cH;D2;+0:12]:1>>[C;D1;H3:5]-[c:6]1:[#7;a:7]:[c:8](:[c:9]):[c:10](:[c:11]):[c;H0;D3;+0:12]:1-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
64.2
[{"value": 64.2, "product": "BrC1=CC=C(CC2=C(NC3=CC(=CC=C23)S(=O)(=O)C)C)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
30
MINUTE
A solution of 6-methanesulfonyl-2-methyl-1H-indole (112 mg), prepared as described in Example 1 Step 3, in 9 ml CH2Cl2 was treated with p-bromo-benzaldehyde (100 mg) and 0.2 ml TMS-OTf. After cooling to 0° C., 0.26 ml of Et3SiH was added. The solution was stirred for 30 minutes followed by partitioning between EtOAc an...
10.6084/m9.figshare.5104873.v1
null
Aldehyde
null
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.c1ccccc1
Other
C(Cl)Cl
0
0.5
Cc1cc2ccc(S(C)(=O)=O)cc2[nH]1.O=Cc1ccc(Br)cc1>C(Cl)Cl>Cc1[nH]c2cc(S(C)(=O)=O)ccc2c1Cc1ccc(Br)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-523b1051d6cf45ca941f7f0badcea3ce
COC(=O)c1cc2ccc(S(C)(=O)=O)cc2[nH]1.Fc1ccc(S)c(F)c1>>COC(=O)c1[nH]c2cc(S(C)(=O)=O)ccc2c1Sc1ccc(F)cc1F
C1=CC=C(C=C1)I(OC(=O)C(F)(F)F)OC(=O)C(F)(F)F.C(=O)(OC)C=1NC2=CC(=CC=C2C1)S(=O)(=O)C.FC1=C(C=CC(=C1)F)S>>COC(=O)C=1NC2=CC(=CC=C2C1SC1=C(C=C(C=C1)F)F)S(=O)(=O)C
[CH3:1][O:2][C:3](=[O:4])[c:5]1[nH:6][c:7]2[cH:8][c:9]([S:10]([CH3:11])(=[O:12])=[O:13])[cH:14][cH:15][c:16]2[cH:17]1.[SH:18][c:19]1[cH:20][cH:21][c:22]([F:23])[cH:24][c:25]1[F:26]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[nH:6][c:7]2[cH:8][c:9]([S:10]([CH3:11])(=[O:12])=[O:13])[cH:14][cH:15][c:16]2[c:17]1[S:18][c:19]1[cH:20][c...
COC(=O)c1cc2ccc(S(C)(=O)=O)cc2[nH]1.Fc1ccc(S)c(F)c1
COC(=O)c1[nH]c2cc(S(C)(=O)=O)ccc2c1Sc1ccc(F)cc1F
null
null
FC(C(C(F)(F)F)O)(F)F
Heteroatom Alkylation and Arylation
OtherReaction
6d0ae58eb1269904d7dda169c1c9a22d9d8065e25d20aca85acf2d11bcd1657c
a20e50d7df818b91ffc2e826d304ad74f6246978a284c599e867e2d806b7437e
c1ccc(Sc2c[nH]c3ccccc23)cc1
[C;D1;H3:1]-[#8:2]-[C:3](=[O;D1;H0:4])-[c:5]1:[#7;a:6]:[c:7](:[c:8]):[c:9](:[c:10]):[cH;D2;+0:11]:1.[SH;D1;+0:12]-[c:13](:[c:14]):[c:15]>>[C;D1;H3:1]-[#8:2]-[C:3](=[O;D1;H0:4])-[c:5]1:[#7;a:6]:[c:7](:[c:8]):[c:9](:[c:10]):[c;H0;D3;+0:11]:1-[S;H0;D2;+0:12]-[c:13](:[c:14]):[c:15]
88
[{"value": 88.0, "product": "COC(=O)C=1NC2=CC(=CC=C2C1SC1=C(C=C(C=C1)F)F)S(=O)(=O)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
A solution of 2-carbomethoxy-6-methylsulfonylindole (750 mg, 2.8 mmol), in 10 mL hexafluoroisopropanol was treated with 2,4-difluorothiophenol (7.5 mmol) followed by addition of PIFA (5.6 mmol). The dark colored solution was stirred overnight then partitioned between methylene chloride and water. After concentration of...
10.6084/m9.figshare.5104873.v1
null
Aromatic thiol
Monosulfide
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.c1ccccc1
null
FC(C(C(F)(F)F)O)(F)F
null
8
COC(=O)c1cc2ccc(S(C)(=O)=O)cc2[nH]1.Fc1ccc(S)c(F)c1>FC(C(C(F)(F)F)O)(F)F>COC(=O)c1[nH]c2cc(S(C)(=O)=O)ccc2c1Sc1ccc(F)cc1F
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-f50514f92a8942ea84682d04f1ea7827
CC(=O)CCl.Oc1ccc(F)cc1>>CC(=O)COc1ccc(F)cc1
FC1=CC=C(C=C1)O.C(=O)([O-])[O-].[K+].[K+].ClCC(C)=O>>FC1=CC=C(OCC(C)=O)C=C1
Cl[CH2:4][C:2]([CH3:1])=[O:3].[OH:5][c:6]1[cH:7][cH:8][c:9]([F:10])[cH:11][cH:12]1>>[CH3:1][C:2](=[O:3])[CH2:4][O:5][c:6]1[cH:7][cH:8][c:9]([F:10])[cH:11][cH:12]1
CC(=O)CCl.Oc1ccc(F)cc1
CC(=O)COc1ccc(F)cc1
null
null
CC(=O)C
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
8060b8e1565497a5ddf79be1adfe74f552b31798797b8841753247b06bdd2051
8749b179916f131d393264a24309227dc6177f560726bed2d1f4567dc2ac63f5
c1ccccc1
Cl-[CH2;D2;+0:1]-[C:2](-[C;D1;H3:3])=[O;D1;H0:4].[OH;D1;+0:5]-[c:6](:[c:7]):[c:8]>>[C;D1;H3:3]-[C:2](=[O;D1;H0:4])-[CH2;D2;+0:1]-[O;H0;D2;+0:5]-[c:6](:[c:7]):[c:8]
null
[]
null
null
8
HOUR
To a mixture of para-fluorophenol (15 g) and K2CO3 (18.5 g) in 100 mL acetone were added chloroacetone (10.4 mL) and of KI (22 g). After heating at reflux for 18 h the reaction mixture was cooled down and left at RT overnight. The reaction mixture was filtered, washed with acetone, and evaporated to dryness. The residu...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ketone.Aromatic alcohol
Ketone.Ether
null
null
c1ccccc1
HCl
CC(=O)C
null
8
CC(=O)CCl.Oc1ccc(F)cc1>CC(=O)C>CC(=O)COc1ccc(F)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-698f412e4a8d4e62afb33c8aea4ddfd7
CS(=O)(=O)c1cccc(N)c1.NN>>CS(=O)(=O)c1cccc(NN)c1
[OH-].[Na+].Cl.NN.CS(=O)(=O)C=1C=C(C=CC1)N.N(=O)[O-].[Na+]>>CS(=O)(=O)C=1C=C(C=CC1)NN
[CH3:1][S:2](=[O:3])(=[O:4])[c:5]1[cH:6][cH:7][cH:8][c:9]([NH2:10])[cH:12]1.N[NH2:11]>>[CH3:1][S:2](=[O:3])(=[O:4])[c:5]1[cH:6][cH:7][cH:8][c:9]([NH:10][NH2:11])[cH:12]1
CS(=O)(=O)c1cccc(N)c1.NN
CS(=O)(=O)c1cccc(NN)c1
null
null
Cl.O
Miscellaneous
OtherReaction
bff6efaab43fcaa1734c9c2b1bb92dedefa785fd0e1362752739094a114b1a2d
edabab25c27777c2204ef93ae7e0a2367d16ed129319c92fb41548ddcbd38608
c1ccccc1
N-[NH2;D1;+0:1].[NH2;D1;+0:2]-[c:3](:[c:4]):[c:5]>>[NH2;D1;+0:1]-[NH;D2;+0:2]-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
To a solution of 3-methanesulphonyl-phenylamine (2.5 g) in 6 mL HCl was added a solution of NaNO2 in 5 mL of H2O at −5° to 0° C. After stirring for 30 min the resulted diazonium salt was poured into a cold solution (−10° to −15° C.) of stannous chloride in 6 ml HCl. The mixture of resulted hydrazine hydrochloride in HC...
10.6084/m9.figshare.5104873.v1
null
Hydrazine.Primary amine
Hydrazine
null
null
c1ccccc1
Other
Cl.O
null
null
CS(=O)(=O)c1cccc(N)c1.NN>Cl.O>CS(=O)(=O)c1cccc(NN)c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-610953b7741c49478a542ec730931570
CC(=O)COc1ccc(F)cc1.CS(=O)(=O)c1cccc(NN)c1>>Cc1[nH]c2cc(S(C)(=O)=O)ccc2c1Oc1ccc(F)cc1
CS(=O)(=O)C=1C=C(C=CC1)NN.FC1=CC=C(OCC(C)=O)C=C1.P(Cl)(Cl)Cl>>FC1=CC=C(OC2=C(NC3=CC(=CC=C23)S(=O)(=O)C)C)C=C1
O=[C:2]([CH3:1])[CH2:14][O:15][c:16]1[cH:17][cH:18][c:19]([F:20])[cH:21][cH:22]1.N[NH:3][c:4]1[cH:5][c:6]([S:7]([CH3:8])(=[O:9])=[O:10])[cH:11][cH:12][cH:13]1>>[CH3:1][c:2]1[nH:3][c:4]2[cH:5][c:6]([S:7]([CH3:8])(=[O:9])=[O:10])[cH:11][cH:12][c:13]2[c:14]1[O:15][c:16]1[cH:17][cH:18][c:19]([F:20])[cH:21][cH:22]1
CC(=O)COc1ccc(F)cc1.CS(=O)(=O)c1cccc(NN)c1
Cc1[nH]c2cc(S(C)(=O)=O)ccc2c1Oc1ccc(F)cc1
null
null
C1=CC=CC=C1
Aromatic Heterocycle Formation
OtherReaction
f7004f13d83fee2783d4405fc57f46a9ac4daac0e3d626cdfc660b16a341e646
0dd0032584e8b699a0d6138c5791ba9322ca70e5c435edc5f54b9d71f78dbd00
c1ccc(Oc2c[nH]c3ccccc23)cc1
N-[NH;D2;+0:1]-[c:2](:[c:3]):[cH;D2;+0:4]:[c:5]:[c:6].O=[C;H0;D3;+0:7](-[C;D1;H3:8])-[CH2;D2;+0:9]-[#8:10]-[c:11]>>[C;D1;H3:8]-[c;H0;D3;+0:7]1:[nH;D2;+0:1]:[c:2](:[c:3]):[c;H0;D3;+0:4](:[c:5]:[c:6]):[c;H0;D3;+0:9]:1-[#8:10]-[c:11]
5.2
[{"value": 5.2, "product": "FC1=CC=C(OC2=C(NC3=CC(=CC=C23)S(=O)(=O)C)C)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To the solution of (3-methanesulfonyl-phenyl)-hydrazine (1.35 g) and 1-(4-fluoro-phenoxy)-propan-2-one (1.01 g) in benzene at RT was added equimolar amount of PCl3. The reaction mixture was stirred at RT for 1 hour and the solvent was removed in vacuo. The residue was purified by Biotage chromatography, eluted with 10–...
10.6084/m9.figshare.5104873.v1
null
Hydrazine.Ketone.Ether
Ether
c1ccccc1
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.c1ccccc1
HO-
C1=CC=CC=C1
null
1
CC(=O)COc1ccc(F)cc1.CS(=O)(=O)c1cccc(NN)c1>C1=CC=CC=C1>Cc1[nH]c2cc(S(C)(=O)=O)ccc2c1Oc1ccc(F)cc1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-30fdb0db690a400e91fadac5b22e9af3
CS(=O)(=O)Cl.CS(=O)(=O)c1ccc2c(Sc3ccccc3Cl)c(CO)[nH]c2c1>>CS(=O)(=O)Cc1[nH]c2cc(S(C)(=O)=O)ccc2c1Sc1ccccc1Cl
CN(C)C=O.CCN(CC)CC.ClC1=C(C=CC=C1)SC1=C(NC2=CC(=CC=C12)S(=O)(=O)C)CO.CS(=O)(=O)Cl>>ClC1=C(C=CC=C1)SC1=C(NC2=CC(=CC=C12)S(=O)(=O)C)CS(=O)(=O)C
Cl[S:2]([CH3:1])(=[O:3])=[O:4].O[CH2:5][c:6]1[nH:7][c:8]2[cH:9][c:10]([S:11]([CH3:12])(=[O:13])=[O:14])[cH:15][cH:16][c:17]2[c:18]1[S:19][c:20]1[cH:21][cH:22][cH:23][cH:24][c:25]1[Cl:26]>>[CH3:1][S:2](=[O:3])(=[O:4])[CH2:5][c:6]1[nH:7][c:8]2[cH:9][c:10]([S:11]([CH3:12])(=[O:13])=[O:14])[cH:15][cH:16][c:17]2[c:18]1[S:19...
CS(=O)(=O)Cl.CS(=O)(=O)c1ccc2c(Sc3ccccc3Cl)c(CO)[nH]c2c1
CS(=O)(=O)Cc1[nH]c2cc(S(C)(=O)=O)ccc2c1Sc1ccccc1Cl
null
null
C(Cl)Cl
Acylation
OtherReaction
0ac8a603953c98c1814574689e0056190c62616c176b8b4c31c7acd96ef43528
7d02e147285bb417922c236d16ce79bf71b54bc3f6dc1c2237422f2069c2cc63
c1ccc(Sc2c[nH]c3ccccc23)cc1
Cl-[S;H0;D4;+0:1](-[C;D1;H3:2])(=[O;D1;H0:3])=[O;D1;H0:4].O-[CH2;D2;+0:5]-[c:6](:[c:7]):[#7;a:8]:[c:9]>>[C;D1;H3:2]-[S;H0;D4;+0:1](=[O;D1;H0:3])(=[O;D1;H0:4])-[CH2;D2;+0:5]-[c:6](:[c:7]):[#7;a:8]:[c:9]
null
[]
null
null
10
MINUTE
[3-(2-chloro-phenylsulfanyl)-6-methanesulfonyl-1H-indol-2-yl]-methanol (1 mmole) (as prepared in Example 5) was dissolved in 2 mL CH2Cl2 and treated with 0.3 mL NEt3 followed by 0.08 ml MsCl. After stirring 10 min. 3 mL DMF was added followed by 0.5 g NaSO2Me. The mixture was stirred overnight. The reaction mixture was...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Sulfonyl halide
Sulfone
null
null
c1ccc2[nH]ccc2c1.c1ccccc1
HCl
C(Cl)Cl
null
0.166667
CS(=O)(=O)Cl.CS(=O)(=O)c1ccc2c(Sc3ccccc3Cl)c(CO)[nH]c2c1>C(Cl)Cl>CS(=O)(=O)Cc1[nH]c2cc(S(C)(=O)=O)ccc2c1Sc1ccccc1Cl
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-2ae93c12a81d411fb6521d083ccbeaea
CS(=O)(=O)c1ccc2c(Sc3ccccc3)c(CO)[nH]c2c1.O=C(Cl)C(=O)Cl>>CS(=O)(=O)c1ccc2c(Sc3ccccc3Cl)c(C=O)[nH]c2c1
C(C)N(CC)CC.CS(=O)(=O)C1=CC=C2C(=C(NC2=C1)CO)SC1=CC=CC=C1.CS(=O)C.C(C(=O)Cl)(=O)Cl>>ClC1=C(C=CC=C1)SC1=C(NC2=CC(=CC=C12)S(=O)(=O)C)C=O
[CH3:1][S:2](=[O:3])(=[O:4])[c:5]1[cH:6][cH:7][c:8]2[c:9]([S:10][c:11]3[cH:12][cH:13][cH:14][cH:15][cH:16]3)[c:18]([CH2:19][OH:20])[nH:21][c:22]2[cH:23]1.O=C(Cl)C(=O)[Cl:17]>>[CH3:1][S:2](=[O:3])(=[O:4])[c:5]1[cH:6][cH:7][c:8]2[c:9]([S:10][c:11]3[cH:12][cH:13][cH:14][cH:15][c:16]3[Cl:17])[c:18]([CH:19]=[O:20])[nH:21][c...
CS(=O)(=O)c1ccc2c(Sc3ccccc3)c(CO)[nH]c2c1.O=C(Cl)C(=O)Cl
CS(=O)(=O)c1ccc2c(Sc3ccccc3Cl)c(C=O)[nH]c2c1
null
null
C(Cl)Cl
Acylation
OtherReaction
977131743567ce3e393f5f6884a1bc719dbe0b0f509fce2ae235f5e2d86155b1
d4f6de1ccba455daea3295211e2abcf26570ce1f4d081f21ccb444a5cef35368
c1ccc(Sc2c[nH]c3ccccc23)cc1
Cl-C(=O)-C(=O)-[Cl;H0;D1;+0:1].[OH;D1;+0:2]-[CH2;D2;+0:3]-[c:4](:[#7;a:5]:[c:6]):[c:7]-[#16:8]-[c:9](:[c:10]):[cH;D2;+0:11]:[c:12]:[c:13]>>[Cl;H0;D1;+0:1]-[c;H0;D3;+0:11](:[c:12]:[c:13]):[c:9](-[#16:8]-[c:7]:[c:4](-[CH;D2;+0:3]=[O;H0;D1;+0:2]):[#7;a:5]:[c:6]):[c:10]
null
[]
null
null
null
null
A solution of alcohol [3-(2-chloro-phenylsulfanyl)-6-methanesulfonyl-1H-indol-2-yl]-methanol (75 mg) (prepared as described in Example 5) in CH2Cl2 (5 ml) was added to a solution of DMSO (0.2 ml) and oxalyl chloride (0.1 ml) that had been prepared at −78°. After 15 min triethylamine (0.45 ml) was added and the reaction...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Acyl halide.Primary alcohol
Aromatic halide.Aldehyde
c1ccccc1
c1ccccc1
c1ccccc1.c1ccc2[nH]ccc2c1
HCl
C(Cl)Cl
null
null
CS(=O)(=O)c1ccc2c(Sc3ccccc3)c(CO)[nH]c2c1.O=C(Cl)C(=O)Cl>C(Cl)Cl>CS(=O)(=O)c1ccc2c(Sc3ccccc3Cl)c(C=O)[nH]c2c1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-1c5a13dd0dcf440dbcd2da5397634bd9
C/C(=N\[Si](C)(C)C)O[Si](C)(C)C.N#Cc1ccc([N+](=O)[O-])cc1.O=S(=O)(Cl)c1cccs1>>O=S(=O)(NCC(CO)c1ccccc1)c1cccs1
[N+](=O)([O-])C1=CC=C(C=C1)C#N.CN1CCOCC1.S1C(=CC=C1)S(=O)(=O)Cl.C/C(=N\[Si](C)(C)C)/O[Si](C)(C)C>>OCC(CNS(=O)(=O)C=1SC=CC1)C1=CC=CC=C1
C[Si](C)(C)/[N:4]=[C:6](\[CH3:5])[O:8][Si](C)(C)C.N#C[c:9]1[cH:10][cH:11][c:12]([N+](=O)[O-])[cH:13][cH:14]1.Cl[S:2](=[O:1])(=[O:3])[c:15]1[cH:16][cH:17][cH:18][s:19]1>>[O:1]=[S:2](=[O:3])([NH:4][CH2:5][CH:6]([CH2:7][OH:8])[c:9]1[cH:10][cH:11][cH:12][cH:13][cH:14]1)[c:15]1[cH:16][cH:17][cH:18][s:19]1
C/C(=N\[Si](C)(C)C)O[Si](C)(C)C.N#Cc1ccc([N+](=O)[O-])cc1.O=S(=O)(Cl)c1cccs1
O=S(=O)(NCC(CO)c1ccccc1)c1cccs1
null
null
O.CC(C)(C)OC.C1CCOC1
Acylation
OtherReaction
266d72bb5a41bebd7073d5c50c7d2737ca37a3157db4c9a314755a78e9640642
b3d053a1893b5f94ac79bc8d06f67773b7e3aea3d0b8779497cdc92075ed3b0c
O=S(=O)(NCCc1ccccc1)c1cccs1
C-[Si](-C)(-C)/[N;H0;D2;+0:1]=[C;H0;D3;+0:2](\[CH3;D1;+0:3])-[O;H0;D2;+0:4]-[Si](-C)(-C)-C.Cl-[S;H0;D4;+0:5](=[O;D1;H0:6])(=[O;D1;H0:7])-[c:8](:[c:9]):[#16;a:10]:[c:11].N#C-[c;H0;D3;+0:12]1:[c:13]:[c:14]:[c;H0;D3;+0:15](-[N+](=O)-[O-]):[c:16]:[c:17]:1>>[O;D1;H0:6]=[S;H0;D4;+0:5](=[O;D1;H0:7])(-[NH;D2;+0:1]-[CH2;D2;+0:3...
83
[{"value": 83.0, "product": "OCC(CNS(=O)(=O)C=1SC=CC1)C1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}]
25
CELSIUS
null
null
A three-necked round bottom flask equipped with a thermocouple, a nitrogen inlet, and a mechanical stirrer was charged with (R)-3-[N-(1-hydroxymethyl-2-phenylethyl)amino]methyl]-4-nitrobenzenecarbonitrile (25 g, 0.08 moles), THF (20 ml), and N-methyl morpholine (NMM) (17.8 mL, 2.0 eq). To this mixture was added N,O-bis...
10.6084/m9.figshare.5104873.v1
null
Nitrile.Nitro group.Sulfonyl halide.Silyl protective group.Silyl protective group
Sulfonamide.Primary alcohol
c1ccccc1
c1ccccc1
c1ccccc1.c1ccsc1
HCl
O.CC(C)(C)OC.C1CCOC1
25
null
C/C(=N\[Si](C)(C)C)O[Si](C)(C)C.N#Cc1ccc([N+](=O)[O-])cc1.O=S(=O)(Cl)c1cccs1>O.CC(C)(C)OC.C1CCOC1>O=S(=O)(NCC(CO)c1ccccc1)c1cccs1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-4cfd76072bfd4a1c94c3b2d643eab6cf
CC(C)(O)C(=O)[O-].ClCC1CO1>>CC(C)(O)C(=O)OCC1CO1
OC(C(=O)[O-])(C)C.[Na+].C(Cl)C1CO1>>OC(C(=O)OCC1CO1)(C)C
[CH3:1][C:2]([CH3:3])([OH:4])[C:5](=[O:6])[O-:7].Cl[CH2:8][CH:9]1[CH2:10][O:11]1>>[CH3:1][C:2]([CH3:3])([OH:4])[C:5](=[O:6])[O:7][CH2:8][CH:9]1[CH2:10][O:11]1
CC(C)(O)C(=O)[O-].ClCC1CO1
CC(C)(O)C(=O)OCC1CO1
null
[Cl-].C[N+](C)(C)C
O
Heteroatom Alkylation and Arylation
OtherReaction
c07f6f64ff82321b3607467d1ee707cb9bab7ac0cd7c3098b7f6ee7c8546417e
670c5cfed3b5aa12e0b1c180fc6f2dc23f2114806bdb54cf3b29925a677cc9b5
C1CO1
Cl-[CH2;D2;+0:1]-[C:2]1-[#8:3]-[C:4]-1.[C:5]-[C:6](-[O-;H0;D1:7])=[O;D1;H0:8]>>[C:5]-[C:6](=[O;D1;H0:8])-[O;H0;D2;+0:7]-[CH2;D2;+0:1]-[C:2]1-[#8:3]-[C:4]-1
null
[]
120
CELSIUS
1.5
HOUR
Into a 200 mL three-necked flask equipped with a stirrer and reflux tube was charged 37.83 g (0.3 mol) of sodium 2-hydroxyisobutyrate, 138.7 g (1.5 mol) of epichlorohydrin, 0.25 g of tetramethylammonium chloride and pure water at room temperature under normal pressure, and heated at temperatures from room temperature t...
10.6084/m9.figshare.5104873.v1
null
Primary halide
Ester
null
null
C1CO1
Other
[Cl-].C[N+](C)(C)C.O
120
1.5
CC(C)(O)C(=O)[O-].ClCC1CO1>[Cl-].C[N+](C)(C)C.O>CC(C)(O)C(=O)OCC1CO1
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-399cca0fbbf6451b89afcb477ad98cfd
CC(C)(C)[Si](C)(C)O[C@@H]1CC2=CC=C3[C@H](CC[C@]4(C)C(CO)=CC[C@@H]34)[C@@]2(C)[C@@H](O[Si](C)(C)C(C)(C)C)C1.CC([O-])=S>>CC(=O)SCC1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C
CS(=O)(=O)Cl.C(C)(=S)[O-].[K+].[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C([C@@]4(C)CC[C@@H]3[C@@]12C)CO)O[Si](C)(C)C(C)(C)C.C(C)N(CC)CC>>C(C)(=O)SCC=1[C@]2(C)[C@@H](CC1)C1=CC=C3C[C@H](C[C@@H]([C@]3(C)[C@H]1CC2)O[Si](C)(C)C(C)(C)C)O[Si](C)(C)C(C)(C)C
O[CH2:5][C:6]1=[CH:7][CH2:8][C@H:9]2[C:10]3=[CH:11][CH:12]=[C:13]4[CH2:14][C@@H:15]([O:16][Si:17]([CH3:18])([CH3:19])[C:20]([CH3:21])([CH3:22])[CH3:23])[CH2:24][C@H:25]([O:26][Si:27]([CH3:28])([CH3:29])[C:30]([CH3:31])([CH3:32])[CH3:33])[C@:34]4([CH3:35])[C@H:36]3[CH2:37][CH2:38][C@:39]12[CH3:40].[CH3:1][C:2]([O-:3])=[...
CC(C)(C)[Si](C)(C)O[C@@H]1CC2=CC=C3[C@H](CC[C@]4(C)C(CO)=CC[C@@H]34)[C@@]2(C)[C@@H](O[Si](C)(C)C(C)(C)C)C1.CC([O-])=S
CC(=O)SCC1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C
null
null
O1CCCC1.CCCCCC.CS(=O)C
Acylation
OtherReaction
f0ef48ecf2991802b01fab2c99f81aa4ec5b243bec9eedcaaebf72a3cffee580
e483c239103a312878e017a96b05cdd3919bff7fb9afe11e6eb3dea046fbf05c
C1=CC2CC[C@H]3C(=CC=C4CCCCC43)[C@@H]2C1
O-[CH2;D2;+0:1]-[C:2](=[C:3]-[C:4])-[C:5].[C;D1;H3:6]-[C;H0;D3;+0:7](-[O-;H0;D1:8])=[S;H0;D1;+0:9]>>[C:5]-[C:2](-[CH2;D2;+0:1]-[S;H0;D2;+0:9]-[C;H0;D3;+0:7](-[C;D1;H3:6])=[O;H0;D1;+0:8])=[C:3]-[C:4]
88.3
[{"value": 88.0, "product": "C(C)(=O)SCC=1[C@]2(C)[C@@H](CC1)C1=CC=C3C[C@H](C[C@@H]([C@]3(C)[C@H]1CC2)O[Si](C)(C)C(C)(C)C)O[Si](C)(C)C(C)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 88.3, "product": "C(C)(=O)SCC=1[C@]2(C)[C@@H](CC1)C1=CC=C3C[C@H](C[C@@H]([C@]3(C)[C@H]1CC2)O[Si](C)(C)C(C)(C)C)O[Si](...
null
null
20
MINUTE
To a solution of 1α,3β-bis(tert-butyldimethylsilyloxy)-17-(hydroxymethyl)androsta-5,7,16-triene (4.00 g, 7.34 mmol) in tetrahydrofuran (70 ml), was added triethylamine (4.10 ml, 29.4 mmol), followed by the dropwise addition of methanesulfonyl chloride (1.70 ml, 22.0 mmol) at −10° C. and stirring for 20 min. The reactio...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Thiocarbonyl
Carbo-thioester
null
null
C1=C[C@H]2CC[C@H]3C(=CC=C4CCCC[C@@H]43)[C@@H]2C1
HO-
O1CCCC1.CCCCCC.CS(=O)C
null
0.333333
CC(C)(C)[Si](C)(C)O[C@@H]1CC2=CC=C3[C@H](CC[C@]4(C)C(CO)=CC[C@@H]34)[C@@]2(C)[C@@H](O[Si](C)(C)C(C)(C)C)C1.CC([O-])=S>O1CCCC1.CCCCCC.CS(=O)C>CC(=O)SCC1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-068d92d58af1432dad376d55043050cc
CC(C)(C)[Si](C)(C)O[C@@H]1CC2=CC=C3[C@H](CC[C@]4(C)C(CBr)=CC[C@@H]34)[C@@]2(C)[C@@H](O[Si](C)(C)C(C)(C)C)C1.CC([O-])=S>>CC(=O)SCC1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C
[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C([C@@]4(C)CC[C@@H]3[C@@]12C)CBr)O[Si](C)(C)C(C)(C)C.C(C)(=S)[O-].[K+]>>C(C)(=O)SCC=1[C@]2(C)[C@@H](CC1)C1=CC=C3C[C@H](C[C@@H]([C@]3(C)[C@H]1CC2)O[Si](C)(C)C(C)(C)C)O[Si](C)(C)C(C)(C)C
Br[CH2:5][C:6]1=[CH:7][CH2:8][C@H:9]2[C:10]3=[CH:11][CH:12]=[C:13]4[CH2:14][C@@H:15]([O:16][Si:17]([CH3:18])([CH3:19])[C:20]([CH3:21])([CH3:22])[CH3:23])[CH2:24][C@H:25]([O:26][Si:27]([CH3:28])([CH3:29])[C:30]([CH3:31])([CH3:32])[CH3:33])[C@:34]4([CH3:35])[C@H:36]3[CH2:37][CH2:38][C@:39]12[CH3:40].[CH3:1][C:2]([O-:3])=...
CC(C)(C)[Si](C)(C)O[C@@H]1CC2=CC=C3[C@H](CC[C@]4(C)C(CBr)=CC[C@@H]34)[C@@]2(C)[C@@H](O[Si](C)(C)C(C)(C)C)C1.CC([O-])=S
CC(=O)SCC1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C
null
null
CCCCCC.CC(=O)C
Acylation
OtherReaction
1f876542c8a2de0f0c93c1e55257e1922650fd69ea48617e41a961445109d4b2
00ab4047825d93b84a3dc255ab210414ba88fbe19a5ef7a3657605acca13230b
C1=CC2CC[C@H]3C(=CC=C4CCCCC43)[C@@H]2C1
Br-[CH2;D2;+0:1]-[C:2](=[C:3]-[C:4])-[C:5].[C;D1;H3:6]-[C;H0;D3;+0:7](-[O-;H0;D1:8])=[S;H0;D1;+0:9]>>[C:5]-[C:2](-[CH2;D2;+0:1]-[S;H0;D2;+0:9]-[C;H0;D3;+0:7](-[C;D1;H3:6])=[O;H0;D1;+0:8])=[C:3]-[C:4]
64
[{"value": 64.0, "product": "C(C)(=O)SCC=1[C@]2(C)[C@@H](CC1)C1=CC=C3C[C@H](C[C@@H]([C@]3(C)[C@H]1CC2)O[Si](C)(C)C(C)(C)C)O[Si](C)(C)C(C)(C)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
To a solution of 1α,3β-bis(tert-butyldimethylsilyloxy)-17-(hydroxymethyl)androsta-5,7,16-triene (100 mg, 0.183 mmol), triphenylphosphine (96.0 mg, 0.366 mmol) and imidazole (49.8 mg, 0.732 mmol) in dichloromethane (2 ml), was added N-bromosuccinimide (65.1 mg, 0.366 mmol) at 0° C., followed by stirring at room temperat...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Thiocarbonyl
Carbo-thioester
null
null
C1=C[C@H]2CC[C@H]3C(=CC=C4CCCC[C@@H]43)[C@@H]2C1
Br-
CCCCCC.CC(=O)C
null
0.5
CC(C)(C)[Si](C)(C)O[C@@H]1CC2=CC=C3[C@H](CC[C@]4(C)C(CBr)=CC[C@@H]34)[C@@]2(C)[C@@H](O[Si](C)(C)C(C)(C)C)C1.CC([O-])=S>CCCCCC.CC(=O)C>CC(=O)SCC1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-9cc781dd66fd4b36b6a7e6f6c86e2e78
CC(C)(C)[Si](C)(C)O[C@@H]1CC2=CC=C3[C@H](CC[C@]4(C)C(CO)=CC[C@@H]34)[C@@]2(C)[C@@H](O[Si](C)(C)C(C)(C)C)C1.CC[Si](CC)(CC)OC(C)(C)CCCBr>>CC[Si](CC)(CC)OC(C)(C)CCCOCC1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C
[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C([C@@]4(C)CC[C@@H]3[C@@]12C)CO)O[Si](C)(C)C(C)(C)C.[H-].[Na+].C1COCCOCCOCCOCCO1.BrCCCC(C)(O[Si](CC)(CC)CC)C>>[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C([C@@]4(C)CC[C@@H]3[C@@]12C)COCCCC(C)(C)O[Si](CC)(CC)CC)O[Si](C)(C)C(C)(C)C
[OH:15][CH2:16][C:17]1=[CH:18][CH2:19][C@H:20]2[C:21]3=[CH:22][CH:23]=[C:24]4[CH2:25][C@@H:26]([O:27][Si:28]([CH3:29])([CH3:30])[C:31]([CH3:32])([CH3:33])[CH3:34])[CH2:35][C@H:36]([O:37][Si:38]([CH3:39])([CH3:40])[C:41]([CH3:42])([CH3:43])[CH3:44])[C@:45]4([CH3:46])[C@H:47]3[CH2:48][CH2:49][C@:50]12[CH3:51].Br[CH2:14][...
CC(C)(C)[Si](C)(C)O[C@@H]1CC2=CC=C3[C@H](CC[C@]4(C)C(CO)=CC[C@@H]34)[C@@]2(C)[C@@H](O[Si](C)(C)C(C)(C)C)C1.CC[Si](CC)(CC)OC(C)(C)CCCBr
CC[Si](CC)(CC)OC(C)(C)CCCOCC1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C
null
null
O1CCCC1.O.C(C)(=O)OCC
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
dd3f9c60e1f90d961a7c01d970ae213561355ee1451f276a3b04696e4b6fae5c
46a6e883cf919b4006e69abfdfd883f458f55c08b3200960c6a5b57c4139fbca
C1=CC2CC[C@H]3C(=CC=C4CCCCC43)[C@@H]2C1
Br-[CH2;D2;+0:1]-[C:2]-[C:3].[C:4]-[C:5]=[C:6](-[C:7]-[OH;D1;+0:8])-[C:9]>>[C:3]-[C:2]-[CH2;D2;+0:1]-[O;H0;D2;+0:8]-[C:7]-[C:6](=[C:5]-[C:4])-[C:9]
100
[{"value": 100.0, "product": "[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C([C@@]4(C)CC[C@@H]3[C@@]12C)COCCCC(C)(C)O[Si](CC)(CC)CC)O[Si](C)(C)C(C)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of 1α,3β-bis(tert-butyldimethylsilyloxy)-17-(hydroxymethyl)androsta-5,7,16-triene (200 mg, 0.367 mmol), sodium hydride (60% in oil, 45 mg, 1.125 mmol) and 15-crown-5 (80 mg, 0.363 mmol) in tetrahydrofuran (1 ml), was added 1-bromo-4-methyl-4-(triethylsilyloxy)pentane (220 mg, 0.745 mmol) at room temperatu...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary alcohol
Ether
null
null
C1=C[C@H]2CC[C@H]3C(=CC=C4CCCC[C@@H]43)[C@@H]2C1
HBr
O1CCCC1.O.C(C)(=O)OCC
null
null
CC(C)(C)[Si](C)(C)O[C@@H]1CC2=CC=C3[C@H](CC[C@]4(C)C(CO)=CC[C@@H]34)[C@@]2(C)[C@@H](O[Si](C)(C)C(C)(C)C)C1.CC[Si](CC)(CC)OC(C)(C)CCCBr>O1CCCC1.O.C(C)(=O)OCC>CC[Si](CC)(CC)OC(C)(C)CCCOCC1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-0e7c0aaac82b48a196a7fd936bac8e10
CC(C)(C)[Si](C)(C)O[C@@H]1CC2=CC=C3[C@H](CC[C@]4(C)C(CO)=CC[C@@H]34)[C@@]2(C)[C@@H](O[Si](C)(C)C(C)(C)C)C1.CCC(CC)(CCCBr)O[Si](CC)(CC)CC>>CCC(CC)(CCCOCC1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C)O[Si](CC)(CC)CC
[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C([C@@]4(C)CC[C@@H]3[C@@]12C)CO)O[Si](C)(C)C(C)(C)C.BrCCCC(CC)(O[Si](CC)(CC)CC)CC.[H-].[Na+].C1COCCOCCOCCOCCO1>>[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C([C@@]4(C)CC[C@@H]3[C@@]12C)COCCCC(CC)(O[Si](CC)(CC)CC)CC)O[Si](C)(C)C(C)(C)C
[OH:9][CH2:10][C:11]1=[CH:12][CH2:13][C@H:14]2[C:15]3=[CH:16][CH:17]=[C:18]4[CH2:19][C@@H:20]([O:21][Si:22]([CH3:23])([CH3:24])[C:25]([CH3:26])([CH3:27])[CH3:28])[CH2:29][C@H:30]([O:31][Si:32]([CH3:33])([CH3:34])[C:35]([CH3:36])([CH3:37])[CH3:38])[C@:39]4([CH3:40])[C@H:41]3[CH2:42][CH2:43][C@:44]12[CH3:45].Br[CH2:8][CH...
CC(C)(C)[Si](C)(C)O[C@@H]1CC2=CC=C3[C@H](CC[C@]4(C)C(CO)=CC[C@@H]34)[C@@]2(C)[C@@H](O[Si](C)(C)C(C)(C)C)C1.CCC(CC)(CCCBr)O[Si](CC)(CC)CC
CCC(CC)(CCCOCC1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C)O[Si](CC)(CC)CC
null
null
O1CCCC1
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
dd3f9c60e1f90d961a7c01d970ae213561355ee1451f276a3b04696e4b6fae5c
46a6e883cf919b4006e69abfdfd883f458f55c08b3200960c6a5b57c4139fbca
C1=CC2CC[C@H]3C(=CC=C4CCCCC43)[C@@H]2C1
Br-[CH2;D2;+0:1]-[C:2]-[C:3].[C:4]-[C:5]=[C:6](-[C:7]-[OH;D1;+0:8])-[C:9]>>[C:4]-[C:5]=[C:6](-[C:7]-[O;H0;D2;+0:8]-[CH2;D2;+0:1]-[C:2]-[C:3])-[C:9]
98.4
[{"value": 98.0, "product": "[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C([C@@]4(C)CC[C@@H]3[C@@]12C)COCCCC(CC)(O[Si](CC)(CC)CC)CC)O[Si](C)(C)C(C)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 98.4, "product": "[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C([C@@]4(C)CC[C@@H]3[C@@]...
null
null
null
null
1α,3β-Bis(tert-butyldimethylsilyloxy)-17-(hydroxymethyl)androsta-5,7,16-triene (400 mg, 0.734 mmol), 1-bromo-4-ethyl-4-(triethylsilyloxy)hexane (475 mg, 1.47 mmol), sodium hydride (60% in oil, 88 mg, 2.20 mmol), 15-crown-5 (162 mg, 0.735 mmol) and tetrahydrofuran (1 ml) were subjected to reaction using a procedure simi...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary alcohol
Ether
null
null
C1=C[C@H]2CC[C@H]3C(=CC=C4CCCC[C@@H]43)[C@@H]2C1
HBr
O1CCCC1
null
null
CC(C)(C)[Si](C)(C)O[C@@H]1CC2=CC=C3[C@H](CC[C@]4(C)C(CO)=CC[C@@H]34)[C@@]2(C)[C@@H](O[Si](C)(C)C(C)(C)C)C1.CCC(CC)(CCCBr)O[Si](CC)(CC)CC>O1CCCC1>CCC(CC)(CCCOCC1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C)O[Si](CC)(CC)CC
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-51ebe64bd2154f2b9412ca6ccc7b36e4
CC(C)(C)[Si](C)(C)O[C@@H]1CC2=CC=C3[C@H](CC[C@]4(C)C(CO)=CC[C@@H]34)[C@@]2(C)[C@@H](O[Si](C)(C)C(C)(C)C)C1.CC[Si](CC)(CC)OC(C)(C)CCCCBr>>CC[Si](CC)(CC)OC(C)(C)CCCCOCC1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C
[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C([C@@]4(C)CC[C@@H]3[C@@]12C)CO)O[Si](C)(C)C(C)(C)C.BrCCCCC(C)(C)O[Si](CC)(CC)CC.[H-].[Na+].C1COCCOCCOCCOCCO1>>[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C([C@@]4(C)CC[C@@H]3[C@@]12C)COCCCCC(C)(C)O[Si](CC)(CC)CC)O[Si](C)(C)C(C)(C)C
[OH:16][CH2:17][C:18]1=[CH:19][CH2:20][C@H:21]2[C:22]3=[CH:23][CH:24]=[C:25]4[CH2:26][C@@H:27]([O:28][Si:29]([CH3:30])([CH3:31])[C:32]([CH3:33])([CH3:34])[CH3:35])[CH2:36][C@H:37]([O:38][Si:39]([CH3:40])([CH3:41])[C:42]([CH3:43])([CH3:44])[CH3:45])[C@:46]4([CH3:47])[C@H:48]3[CH2:49][CH2:50][C@:51]12[CH3:52].Br[CH2:15][...
CC(C)(C)[Si](C)(C)O[C@@H]1CC2=CC=C3[C@H](CC[C@]4(C)C(CO)=CC[C@@H]34)[C@@]2(C)[C@@H](O[Si](C)(C)C(C)(C)C)C1.CC[Si](CC)(CC)OC(C)(C)CCCCBr
CC[Si](CC)(CC)OC(C)(C)CCCCOCC1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C
null
null
O1CCCC1
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
dd3f9c60e1f90d961a7c01d970ae213561355ee1451f276a3b04696e4b6fae5c
46a6e883cf919b4006e69abfdfd883f458f55c08b3200960c6a5b57c4139fbca
C1=CC2CC[C@H]3C(=CC=C4CCCCC43)[C@@H]2C1
Br-[CH2;D2;+0:1]-[C:2]-[C:3].[C:4]-[C:5]=[C:6](-[C:7]-[OH;D1;+0:8])-[C:9]>>[C:3]-[C:2]-[CH2;D2;+0:1]-[O;H0;D2;+0:8]-[C:7]-[C:6](=[C:5]-[C:4])-[C:9]
95.1
[{"value": 95.0, "product": "[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C([C@@]4(C)CC[C@@H]3[C@@]12C)COCCCCC(C)(C)O[Si](CC)(CC)CC)O[Si](C)(C)C(C)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 95.1, "product": "[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C([C@@]4(C)CC[C@@H]3[C@@]1...
null
null
null
null
1α,3β-Bis(tert-butyldimethylsilyloxy)-17-(hydroxymethyl)androsta-5,7,16-triene (200 mg, 0.367 mmol), 1-bromo-5-triethylsilyloxy-5-methylhexane (227 mg, 0.734 mmol), sodium hydride (60% in oil, 44 mg, 1.10 mmol), 15-crown-5 (81 mg, 0.368 mmol) and tetrahydrofuran (0.5 ml) were subjected to reaction using a procedure sim...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary alcohol
Ether
null
null
C1=C[C@H]2CC[C@H]3C(=CC=C4CCCC[C@@H]43)[C@@H]2C1
HBr
O1CCCC1
null
null
CC(C)(C)[Si](C)(C)O[C@@H]1CC2=CC=C3[C@H](CC[C@]4(C)C(CO)=CC[C@@H]34)[C@@]2(C)[C@@H](O[Si](C)(C)C(C)(C)C)C1.CC[Si](CC)(CC)OC(C)(C)CCCCBr>O1CCCC1>CC[Si](CC)(CC)OC(C)(C)CCCCOCC1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-bdea4a72c64b44bfae57265ad669ee45
CC(C)(C)[Si](C)(C)O[C@@H]1CC2=CC=C3[C@H](CC[C@]4(C)C(CO)=CC[C@@H]34)[C@@]2(C)[C@@H](O[Si](C)(C)C(C)(C)C)C1.CC[Si](CC)(CC)OC(C)(C)C#CCBr>>CC[Si](CC)(CC)OC(C)(C)C#CCOCC1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C
[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C([C@@]4(C)CC[C@@H]3[C@@]12C)CO)O[Si](C)(C)C(C)(C)C.BrCC#CC(C)(C)O[Si](CC)(CC)CC.[H-].[Na+].C1COCCOCCOCCOCCO1>>[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C([C@@]4(C)CC[C@@H]3[C@@]12C)COCC#CC(C)(C)O[Si](CC)(CC)CC)O[Si](C)(C)C(C)(C)C
[OH:15][CH2:16][C:17]1=[CH:18][CH2:19][C@H:20]2[C:21]3=[CH:22][CH:23]=[C:24]4[CH2:25][C@@H:26]([O:27][Si:28]([CH3:29])([CH3:30])[C:31]([CH3:32])([CH3:33])[CH3:34])[CH2:35][C@H:36]([O:37][Si:38]([CH3:39])([CH3:40])[C:41]([CH3:42])([CH3:43])[CH3:44])[C@:45]4([CH3:46])[C@H:47]3[CH2:48][CH2:49][C@:50]12[CH3:51].Br[CH2:14][...
CC(C)(C)[Si](C)(C)O[C@@H]1CC2=CC=C3[C@H](CC[C@]4(C)C(CO)=CC[C@@H]34)[C@@]2(C)[C@@H](O[Si](C)(C)C(C)(C)C)C1.CC[Si](CC)(CC)OC(C)(C)C#CCBr
CC[Si](CC)(CC)OC(C)(C)C#CCOCC1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C
null
null
O1CCCC1
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
dd3f9c60e1f90d961a7c01d970ae213561355ee1451f276a3b04696e4b6fae5c
46a6e883cf919b4006e69abfdfd883f458f55c08b3200960c6a5b57c4139fbca
C1=CC2CC[C@H]3C(=CC=C4CCCCC43)[C@@H]2C1
Br-[CH2;D2;+0:1]-[C:2]#[C:3]-[C:4].[C:5]-[C:6]=[C:7](-[C:8]-[OH;D1;+0:9])-[C:10]>>[C:5]-[C:6]=[C:7](-[C:8]-[O;H0;D2;+0:9]-[CH2;D2;+0:1]-[C:2]#[C:3]-[C:4])-[C:10]
66
[{"value": 66.0, "product": "[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C([C@@]4(C)CC[C@@H]3[C@@]12C)COCC#CC(C)(C)O[Si](CC)(CC)CC)O[Si](C)(C)C(C)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 66.0, "product": "[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C([C@@]4(C)CC[C@@H]3[C@@]1...
null
null
null
null
1α,3β-Bis(tert-butyldimethylsilyloxy)-17-(hydroxymethyl)androsta-5,7,16-triene (200 mg, 0.367 mmol), 1-bromo-4-triethylsilyloxy-4-methyl-2-pentyne (216 mg, 0.741 mmol), sodium hydride (60% in oil, 44 mg, 1.10 mmol) 15-crown-5 (81 mg, 0.368 mmol) and tetrahydrofuran (1 ml) were subjected to reaction using a procedure si...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary alcohol
Ether
null
null
C1=C[C@H]2CC[C@H]3C(=CC=C4CCCC[C@@H]43)[C@@H]2C1
HBr
O1CCCC1
null
null
CC(C)(C)[Si](C)(C)O[C@@H]1CC2=CC=C3[C@H](CC[C@]4(C)C(CO)=CC[C@@H]34)[C@@]2(C)[C@@H](O[Si](C)(C)C(C)(C)C)C1.CC[Si](CC)(CC)OC(C)(C)C#CCBr>O1CCCC1>CC[Si](CC)(CC)OC(C)(C)C#CCOCC1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-d73a24bb858946d1bbd1c0ffe34a20a8
CC(C)(C)[Si](C)(C)O[C@@H]1CC2=CC=C3[C@H](CC[C@]4(C)C(CO)=CC[C@@H]34)[C@@]2(C)[C@@H](O[Si](C)(C)C(C)(C)C)C1.CC[Si](CC)(CC)OC(C)(C)C/C=C/Br>>CC[Si](CC)(CC)OC(C)(C)C/C=C/OCC1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C
[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C([C@@]4(C)CC[C@@H]3[C@@]12C)CO)O[Si](C)(C)C(C)(C)C.Br\C=C\CC(C)(C)O[Si](CC)(CC)CC.[H-].[Na+].C1COCCOCCOCCOCCO1>>[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C([C@@]4(C)CC[C@@H]3[C@@]12C)CO\C=C\CC(C)(C)O[Si](CC)(CC)CC)O[Si](C)(C)C(C)(C)C
[OH:15][CH2:16][C:17]1=[CH:18][CH2:19][C@H:20]2[C:21]3=[CH:22][CH:23]=[C:24]4[CH2:25][C@@H:26]([O:27][Si:28]([CH3:29])([CH3:30])[C:31]([CH3:32])([CH3:33])[CH3:34])[CH2:35][C@H:36]([O:37][Si:38]([CH3:39])([CH3:40])[C:41]([CH3:42])([CH3:43])[CH3:44])[C@:45]4([CH3:46])[C@H:47]3[CH2:48][CH2:49][C@:50]12[CH3:51].Br/[CH:14]=...
CC(C)(C)[Si](C)(C)O[C@@H]1CC2=CC=C3[C@H](CC[C@]4(C)C(CO)=CC[C@@H]34)[C@@]2(C)[C@@H](O[Si](C)(C)C(C)(C)C)C1.CC[Si](CC)(CC)OC(C)(C)C/C=C/Br
CC[Si](CC)(CC)OC(C)(C)C/C=C/OCC1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C
null
null
O1CCCC1
Acylation
Williamson Ether Synthesis
6ea2ecb1a9662f756e9e0abf21897ef5086f34c2e732d2ef2696caeea95650ca
d81e0d3b4d57ff7b2f3fcadb65b1e8eb90864aba075c535b9ef521dca07670ef
C1=CC2CC[C@H]3C(=CC=C4CCCCC43)[C@@H]2C1
Br/[CH;D2;+0:1]=[C:2]/[C:3]-[C:4].[C:5]-[C:6]=[C:7](-[C:8]-[OH;D1;+0:9])-[C:10]>>[C:5]-[C:6]=[C:7](-[C:8]-[O;H0;D2;+0:9]/[CH;D2;+0:1]=[C:2]/[C:3]-[C:4])-[C:10]
100
[{"value": 100.0, "product": "[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C([C@@]4(C)CC[C@@H]3[C@@]12C)CO\\C=C\\CC(C)(C)O[Si](CC)(CC)CC)O[Si](C)(C)C(C)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 100.0, "product": "[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C([C@@]4(C)CC[C@@H]3...
null
null
null
null
1α,3β-Bis(tert-butyldimethylsilyloxy)-17-(hydroxymethyl)androsta-5,7,16-triene (400 mg, 0.734 mmol), 1-bromo-4-triethylsilyloxy-4-methyl-(2E)-pentene (431 mg, 1.47 mmol), sodium hydride (60% in oil, 88 mg, 2.20 mmol), 15-crown-5 (162 mg, 0.735 mmol) and tetrahydrofuran (1 ml) were subjected to reaction using a procedur...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Ether
null
null
C1=C[C@H]2CC[C@H]3C(=CC=C4CCCC[C@@H]43)[C@@H]2C1
HBr
O1CCCC1
null
null
CC(C)(C)[Si](C)(C)O[C@@H]1CC2=CC=C3[C@H](CC[C@]4(C)C(CO)=CC[C@@H]34)[C@@]2(C)[C@@H](O[Si](C)(C)C(C)(C)C)C1.CC[Si](CC)(CC)OC(C)(C)C/C=C/Br>O1CCCC1>CC[Si](CC)(CC)OC(C)(C)C/C=C/OCC1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C
ord_dataset-c3a75813d0b24864aa4f7cd526efd6aa
ord-181ba1521ec749ff9911042772875c44
CC(C)(O)C1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C.CCC(CC)(CCCBr)O[Si](CC)(CC)CC>>CCC(CC)(CCCOC(C)(C)C1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C)O[Si](CC)(CC)CC
[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C(C(C)(C)O)[C@]4(CC[C@@H]3[C@@]12C)C)O[Si](C)(C)C(C)(C)C.BrCCCC(CC)(O[Si](CC)(CC)CC)CC.[H-].[Na+].C1COCCOCCOCCOCCO1>>[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C(C(C)(C)OCCCC(CC)(O[Si](CC)(CC)CC)CC)[C@]4(CC[C@@H]3[C@@]12C)C)O[Si](C)(C)C(C)(C)C
[OH:9][C:10]([CH3:11])([CH3:12])[C:13]1=[CH:14][CH2:15][C@H:16]2[C:17]3=[CH:18][CH:19]=[C:20]4[CH2:21][C@@H:22]([O:23][Si:24]([CH3:25])([CH3:26])[C:27]([CH3:28])([CH3:29])[CH3:30])[CH2:31][C@H:32]([O:33][Si:34]([CH3:35])([CH3:36])[C:37]([CH3:38])([CH3:39])[CH3:40])[C@:41]4([CH3:42])[C@H:43]3[CH2:44][CH2:45][C@:46]12[CH...
CC(C)(O)C1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C.CCC(CC)(CCCBr)O[Si](CC)(CC)CC
CCC(CC)(CCCOC(C)(C)C1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C)O[Si](CC)(CC)CC
null
null
O1CCCC1
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
9ef84a8c80411e848c10c5384ce78141e473ad5db44b97f46285876278d6d001
004868630acb495c3cf864467df50d8e3d3bf839809342ad5aeae72f8c34f6c8
C1=CC2CC[C@H]3C(=CC=C4CCCCC43)[C@@H]2C1
Br-[CH2;D2;+0:1]-[C:2]-[C:3].[C:4]-[C:5]=[C:6](-[C:7](-[C;D1;H3:8])(-[C;D1;H3:9])-[OH;D1;+0:10])-[C:11]>>[C:4]-[C:5]=[C:6](-[C:7](-[C;D1;H3:8])(-[C;D1;H3:9])-[O;H0;D2;+0:10]-[CH2;D2;+0:1]-[C:2]-[C:3])-[C:11]
100.2
[{"value": 100.0, "product": "[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C(C(C)(C)OCCCC(CC)(O[Si](CC)(CC)CC)CC)[C@]4(CC[C@@H]3[C@@]12C)C)O[Si](C)(C)C(C)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 100.2, "product": "[Si](C)(C)(C(C)(C)C)O[C@H]1C[C@@H](CC2=CC=C3[C@@H]4CC=C(C(C)(C)OCCCC(CC)...
null
null
null
null
1α,3β-Bis(tert-butyldimethylsilyloxy)-20-hydroxy-20-methylpregna-5,7,16-triene (100 mg, 0.175 mmol), 1-bromo-4-ethyl-4-(triethylsilyloxy)hexane (225 mg, 0.696 mmol), sodium hydride (60% in oil, 42 mg, 1.05 mmol), 15-crown-5 (38 mg, 0.173 mmol) and tetrahydrofuran (3 ml) were subjected to reaction using a procedure simi...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Tertiary alcohol
Ether
null
null
C1=C[C@H]2CC[C@H]3C(=CC=C4CCCC[C@@H]43)[C@@H]2C1
HBr
O1CCCC1
null
null
CC(C)(O)C1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C.CCC(CC)(CCCBr)O[Si](CC)(CC)CC>O1CCCC1>CCC(CC)(CCCOC(C)(C)C1=CC[C@H]2C3=CC=C4C[C@@H](O[Si](C)(C)C(C)(C)C)C[C@H](O[Si](C)(C)C(C)(C)C)[C@]4(C)[C@H]3CC[C@]12C)O[Si](CC)(CC)CC