dataset_id
large_stringclasses
414 values
reaction_id
large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
reactant_smiles
large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-1239a307ee3d4a5296ffa6fb6b34bcfc
COC(=O)C#CC(=O)OC.COC(=O)c1c(N)cccc1OC>>COC(=O)c1nc2cccc(OC)c2c(O)c1C(=O)OC
NC1=C(C(=O)OC)C(=CC=C1)OC.C(#CC(=O)OC)C(=O)OC.CC(C)([O-])C.[K+]>>OC1=C(C(=NC2=CC=CC(=C12)OC)C(=O)OC)C(=O)OC
[CH3:1][O:2][C:3](=[O:4])[C:5]#[C:17][C:18](=[O:19])[O:20][CH3:21].CO[C:15]([c:14]1[c:7]([NH2:6])[cH:8][cH:9][cH:10][c:11]1[O:12][CH3:13])=[O:16]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[n:6][c:7]2[cH:8][cH:9][cH:10][c:11]([O:12][CH3:13])[c:14]2[c:15]([OH:16])[c:17]1[C:18](=[O:19])[O:20][CH3:21]
COC(=O)C#CC(=O)OC.COC(=O)c1c(N)cccc1OC
COC(=O)c1nc2cccc(OC)c2c(O)c1C(=O)OC
null
null
C(C)(C)(C)O
Aromatic Heterocycle Formation
OtherReaction
f5368757c96521e83619cf21dfc52b28c31825e0516659832aaa47488ac6716c
bbcf1c85e1dbdba58f5fefc8b60992ba8e370d006abd0aa7780d40fd3f3dc3a2
c1ccc2ncccc2c1
C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3](:[c:4]):[c:5](-[NH2;D1;+0:6]):[c:7].[C;D1;H3:8]-[#8:9]-[C:10](=[O;D1;H0:11])-[C;H0;D2;+0:12]#[C;H0;D2;+0:13]-[C:14](=[O;D1;H0:15])-[#8:16]-[C;D1;H3:17]>>[C;D1;H3:8]-[#8:9]-[C:10](=[O;D1;H0:11])-[c;H0;D3;+0:12]1:[n;H0;D2;+0:6]:[c:5](:[c:7]):[c:3](:[c:4]):[c;H0;D3;+0:1](-[OH;D1;+...
65
[{"value": 65.0, "product": "OC1=C(C(=NC2=CC=CC(=C12)OC)C(=O)OC)C(=O)OC", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of methyl 2-amino-6-methoxybenzoate ((1.30 g, 7.17 mM) and dimethyl acetylenedicarboxylate (1.17 g, 8.23 mM) in t-butanol (11 mL) was refluxed under a nitrogen atmosphere for 4 hr. The reaction mixture was cooled to room temperature, potassium t-butoxide (0.92 g, 8.23 mM) was added, and the resulting mixture...
10.6084/m9.figshare.5104873.v1
null
Ester.Ester.Ester.Primary amine
Ester.Ester.Aromatic alcohol
c1ccccc1
c1ccc2ncccc2c1
c1ccc2ncccc2c1
HO-
C(C)(C)(C)O
null
null
COC(=O)C#CC(=O)OC.COC(=O)c1c(N)cccc1OC>C(C)(C)(C)O>COC(=O)c1nc2cccc(OC)c2c(O)c1C(=O)OC
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-e1f559619b474a8e8ddc858df147e65a
COC(=O)c1nc2cc(Cl)ccc2c(Cl)c1C(=O)OC>>COC(=O)c1cc2ccc(Cl)cc2nc1C(=O)OC
ClC1=C(C(=NC2=CC(=CC=C12)Cl)C(=O)OC)C(=O)OC.C(=O)[O-].[Na+].O>>ClC1=CC=C2C=C(C(=NC2=C1)C(=O)OC)C(=O)OC
Cl[c:6]1[c:5]([C:3]([O:2][CH3:1])=[O:4])[c:15]([C:16](=[O:17])[O:18][CH3:19])[n:14][c:13]2[c:7]1[cH:8][cH:9][c:10]([Cl:11])[cH:12]2>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]2[cH:8][cH:9][c:10]([Cl:11])[cH:12][c:13]2[n:14][c:15]1[C:16](=[O:17])[O:18][CH3:19]
COC(=O)c1nc2cc(Cl)ccc2c(Cl)c1C(=O)OC
COC(=O)c1cc2ccc(Cl)cc2nc1C(=O)OC
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
CN(C=O)C
Functional Group Interconversion
Aromatic dehalogenation
9d8b09641537c9b7067a6060cf65ecd110c7af466a7b229ce3601533f966554e
56de34d4a44cb25d9380269ee5e138b0f24b40a3a0db22c5508049dc775a861f
c1ccc2ncccc2c1
Cl-[c;H0;D3;+0:1]1:[c:2](-[C:3](=[O;D1;H0:4])-[#8:5]-[C;D1;H3:6]):[c:7](-[C:8](-[#8:9])=[O;D1;H0:10]):[#7;a:11]:[c:12](:[c:13]):[c:14]:1:[c:15]>>[#8:9]-[C:8](=[O;D1;H0:10])-[c:7]1:[#7;a:11]:[c:12](:[c:13]):[c:14](:[c:15]):[cH;D2;+0:1]:[c:2]:1-[C:3](=[O;D1;H0:4])-[#8:5]-[C;D1;H3:6]
134.8
[{"value": 134.8, "product": "ClC1=CC=C2C=C(C(=NC2=C1)C(=O)OC)C(=O)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A stirred mixture of dimethyl 4,7-dichloroquinoline-2,3-dicarboxylate (5.00 g, 15.9 mM), sodium formate (1.63 g, 23.9 mM) and tetrakis(triphenylphosphine)palladium(0) (0.92 g, 0.80 mM) in anhydrous dimethylformamide (75 mL) under a nitrogen atmosphere was heated at 90°-95° C. for 7 hr. No reaction occurred so the react...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1ccc2ncccc2c1
c1ccc2ncccc2c1
c1ccc2ncccc2c1
Other
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.CN(C=O)C
null
null
COC(=O)c1nc2cc(Cl)ccc2c(Cl)c1C(=O)OC>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.CN(C=O)C>COC(=O)c1cc2ccc(Cl)cc2nc1C(=O)OC
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-454fe2e70f3f4c0c89014e75840e632f
COC(=O)c1nc2ccccc2c(N)c1C(=O)OC.NN>>Nc1c2ccccc2nc2c(=O)[nH][nH]c(=O)c12
NC1=C(C(=NC2=CC=CC=C12)C(=O)OC)C(=O)OC.O.NN>>NC1=C2C(=NC=3C=CC=CC13)C(NNC2=O)=O
CO[C:11]([c:10]1[n:9][c:8]2[c:3]([c:2]([NH2:1])[c:17]1[C:15](OC)=[O:16])[cH:4][cH:5][cH:6][cH:7]2)=[O:12].[NH2:13][NH2:14]>>[NH2:1][c:2]1[c:3]2[cH:4][cH:5][cH:6][cH:7][c:8]2[n:9][c:10]2[c:11](=[O:12])[nH:13][nH:14][c:15](=[O:16])[c:17]12
COC(=O)c1nc2ccccc2c(N)c1C(=O)OC.NN
Nc1c2ccccc2nc2c(=O)[nH][nH]c(=O)c12
null
null
C(C)O
Aromatic Heterocycle Formation
OtherReaction
ec1917a0188259fb1d502a40ed3d9aad8b3b567f28677d868775be5ee838e719
1775b7eba35fc46eaa0b0ad39cde9e207db465168e4fe5d9832db816e257be74
O=c1[nH][nH]c(=O)c2nc3ccccc3cc12
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[#7;a:4]:[c:5]):[c:6](-[C;H0;D3;+0:7](=[O;D1;H0:8])-O-C):[c:9].[NH2;D1;+0:10]-[NH2;D1;+0:11]>>[O;D1;H0:2]=[c;H0;D3;+0:1]1:[nH;D2;+0:10]:[nH;D2;+0:11]:[c;H0;D3;+0:7](=[O;D1;H0:8]):[c:6](:[c:9]):[c:3]:1:[#7;a:4]:[c:5]
98.8
[{"value": 68.0, "product": "NC1=C2C(=NC=3C=CC=CC13)C(NNC2=O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 98.8, "product": "NC1=C2C(=NC=3C=CC=CC13)C(NNC2=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a stirred solution of dimethyl 4-aminoquinoline-2,3-dicarboxylate (0.15 g, 0.58 mM) in ethanol (4 mL) was added hydrazine hydrate (1.46 g, 29.2 mM) and the resulting solution was refluxed for 3 hr. The reaction mixture was cooled to room temperature and filtered to separate the yellow precipitate (0.12 g). This mate...
10.6084/m9.figshare.5104873.v1
null
Hydrazine.Ester.Ester
null
c1ccc2ncccc2c1
C1=c2cc3ccccc3nc2=CNN1
C1=c2cc3ccccc3nc2=CNN1
HO-
C(C)O
null
null
COC(=O)c1nc2ccccc2c(N)c1C(=O)OC.NN>C(C)O>Nc1c2ccccc2nc2c(=O)[nH][nH]c(=O)c12
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-07ccba316ab64ff1a0c5fdbf401e073f
COC(=O)C#CC(=O)OC.N#Cc1ccccc1N>>COC(=O)/C=C(\Nc1ccccc1C#N)C(=O)OC
NC1=C(C#N)C=CC=C1.C(#CC(=O)OC)C(=O)OC>>C(#N)C1=C(N/C(/C(=O)OC)=C\C(=O)OC)C=CC=C1
[CH3:1][O:2][C:3](=[O:4])[C:5]#[C:6][C:16](=[O:17])[O:18][CH3:19].[NH2:7][c:8]1[cH:9][cH:10][cH:11][cH:12][c:13]1[C:14]#[N:15]>>[CH3:1][O:2][C:3](=[O:4])/[CH:5]=[C:6](\[NH:7][c:8]1[cH:9][cH:10][cH:11][cH:12][c:13]1[C:14]#[N:15])[C:16](=[O:17])[O:18][CH3:19]
COC(=O)C#CC(=O)OC.N#Cc1ccccc1N
COC(=O)/C=C(\Nc1ccccc1C#N)C(=O)OC
null
null
C(C)(C)(C)O
Heteroatom Alkylation and Arylation
OtherReaction
3d5adf24dd93857513fe82642f7d3d4feab92a8bf952edd7458e6f077b54016e
cb45d3f2664ea1c07edca6192a95c91d6c98f4c61196cc5a896d41447e7a94b5
c1ccccc1
[C;D1;H3:1]-[#8:2]-[C:3](=[O;D1;H0:4])-[C;H0;D2;+0:5]#[C;H0;D2;+0:6]-[C:7](=[O;D1;H0:8])-[#8:9]-[C;D1;H3:10].[NH2;D1;+0:11]-[c:12](:[c:13]):[c:14]>>[C;D1;H3:1]-[#8:2]-[C:3](=[O;D1;H0:4])/[C;H0;D3;+0:5](=[CH;D2;+0:6]/[C:7](=[O;D1;H0:8])-[#8:9]-[C;D1;H3:10])-[NH;D2;+0:11]-[c:12](:[c:13]):[c:14]
44.3
[{"value": 44.3, "product": "C(#N)C1=C(N/C(/C(=O)OC)=C\\C(=O)OC)C=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 2-aminobenzonitrile (5.00 g, 42.3 mM) and dimethyl acetylenedicarboxylate (6.42 g, 45.2 mM) in t-butanol (70.5 mL) was refluxed under a nitrogen atmosphere for 12 hr. After cooling the reaction mixture to room temperature, a precipitate formed and was collected by filtration. The material was washed with ...
10.6084/m9.figshare.5104873.v1
null
Ester.Ester.Primary amine
Enamine
null
null
c1ccccc1
null
C(C)(C)(C)O
null
null
COC(=O)C#CC(=O)OC.N#Cc1ccccc1N>C(C)(C)(C)O>COC(=O)/C=C(\Nc1ccccc1C#N)C(=O)OC
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-57ce19bea6534a878ad8a04143464a6c
O.O=C1Nc2cc(I)ccc2C1=O>>O=c1[nH]c2cc(I)ccc2c(=O)o1
IC1=CC=C2C(C(NC2=C1)=O)=O.O>>IC1=CC2=C(C(OC(N2)=O)=O)C=C1
[OH2:13].[O:1]=[C:2]1[NH:3][c:4]2[cH:5][c:6]([I:7])[cH:8][cH:9][c:10]2[C:11]1=[O:12]>>[O:1]=[c:2]1[nH:3][c:4]2[cH:5][c:6]([I:7])[cH:8][cH:9][c:10]2[c:11](=[O:12])[o:13]1
O.O=C1Nc2cc(I)ccc2C1=O
O=c1[nH]c2cc(I)ccc2c(=O)o1
null
[O-2].[O-2].[O-2].[Cr+6]
C(C)(=O)O.C(C)(=O)OC(C)=O
Miscellaneous
OtherReaction
5d9736fd05de108b71c591acfae61cb6af4635bfbe20446a56c7b74a3d5953af
8242b1e5e71ebd9e44538af93284e3a1145dd4183387fabf58d37d4a04b884a5
O=c1[nH]c2ccccc2c(=O)o1
[O;D1;H0:1]=[C;H0;D3;+0:2]1-[C;H0;D3;+0:3](=[O;D1;H0:4])-[NH;D2;+0:5]-[c:6](:[c:7]):[c:8]-1:[c:9].[OH2;D0;+0:10]>>[O;D1;H0:1]=[c;H0;D3;+0:2]1:[o;H0;D2;+0:10]:[c;H0;D3;+0:3](=[O;D1;H0:4]):[nH;D2;+0:5]:[c:6](:[c:7]):[c:8]:1:[c:9]
81.8
[{"value": 81.8, "product": "IC1=CC2=C(C(OC(N2)=O)=O)C=C1", "details": "PERCENTYIELD", "is_desired": false}]
80
CELSIUS
null
null
To a stirred warm (80° C.) solution of 6-iodo-1H-indole-2,3-dione (3.0 g, 11 mM) in acetic acid (10 mL) and acetic anhydride (10 mL) was added in small portions chromium trioxide (1.83 g, 18.3 mM) while maintaining the temperature of the reaction mixture at 80°-90° C. The reaction mixture was then heated at 80° C. for ...
10.6084/m9.figshare.5104873.v1
null
Ketone.Secondary amide
null
c1ccc2c(c1)CCN2
c1ccc2cocnc2c1
c1ccc2cocnc2c1
null
[O-2].[O-2].[O-2].[Cr+6].C(C)(=O)O.C(C)(=O)OC(C)=O
80
null
O.O=C1Nc2cc(I)ccc2C1=O>[O-2].[O-2].[O-2].[Cr+6].C(C)(=O)O.C(C)(=O)OC(C)=O>O=c1[nH]c2cc(I)ccc2c(=O)o1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-c4712f788bc44516bf8778e183920013
O=c1[nH]c2cc(I)ccc2c(=O)o1>>COC(=O)c1ccc(I)cc1N
O.[OH-].[Na+].IC1=CC2=C(C(OC(N2)=O)=O)C=C1>>NC1=C(C(=O)OC)C=CC(=C1)I
O=[c:1]1[o:2][c:3](=[O:4])[c:5]2[cH:6][cH:7][c:8]([I:9])[cH:10][c:11]2[nH:12]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([I:9])[cH:10][c:11]1[NH2:12]
O=c1[nH]c2cc(I)ccc2c(=O)o1
COC(=O)c1ccc(I)cc1N
null
null
CO
Reduction
OtherReaction
fb3a8999d982d1c42a150fbbeb96fa0db2838a9c48a5140f183de4d3421c8ad6
9f87be38aa9793f80b3cef223629015a04ccba30a9633b313486e0a6edc9c43d
c1ccccc1
O=[c;H0;D3;+0:1]1:[nH;D2;+0:2]:[c:3](:[c:4]):[c:5](:[c:6]):[c;H0;D3;+0:7](=[O;D1;H0:8]):[o;H0;D2;+0:9]:1>>[CH3;D1;+0:1]-[O;H0;D2;+0:9]-[C;H0;D3;+0:7](=[O;D1;H0:8])-[c:5](:[c:6]):[c:3](-[NH2;D1;+0:2]):[c:4]
80.2
[{"value": 80.0, "product": "NC1=C(C(=O)OC)C=CC(=C1)I", "details": "PERCENTYIELD", "is_desired": false}, {"value": 80.2, "product": "NC1=C(C(=O)OC)C=CC(=C1)I", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
null
null
To a stirred solution of sodium hydroxide (0.048 g, 1.2 mM) in methanol (4.5 mL) was added 7-iodo-2H-3,1-benzoxazine-2,4(1H)-dione (2.6 g, 9.0 mM). The mixture was heated at 60° C. for 7 hr and the resulting solution was cooled, poured into water and extracted with ethyl acetate. The combined extracts were washed once ...
10.6084/m9.figshare.5104873.v1
null
null
Ester.Primary amine
c1ccc2cocnc2c1
c1ccccc1
c1ccccc1
Other
CO
60
null
O=c1[nH]c2cc(I)ccc2c(=O)o1>CO>COC(=O)c1ccc(I)cc1N
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-ec04a768a81546c687358bb4525e5d24
CCOC(=O)CC(=O)C(=O)OCC.O=c1[nH]c2cc(Br)ccc2c(=O)o1>>CCOC(=O)c1nc2cc(Br)ccc2c(O)c1C(=O)OCC
[Na].O=C(C(=O)OCC)CC(=O)OCC.BrC1=CC2=C(C(OC(N2)=O)=O)C=C1>>BrC1=CC=C2C(=C(C(=NC2=C1)C(=O)OCC)C(=O)OCC)O
O=[C:17]([CH2:6][C:4]([O:3][CH2:2][CH3:1])=[O:5])[C:18](=[O:19])[O:20][CH2:21][CH3:22].O=c1[nH:7][c:8]2[cH:9][c:10]([Br:11])[cH:12][cH:13][c:14]2[c:15](=O)[o:16]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[n:7][c:8]2[cH:9][c:10]([Br:11])[cH:12][cH:13][c:14]2[c:15]([OH:16])[c:17]1[C:18](=[O:19])[O:20][CH2:21][CH3:22]
CCOC(=O)CC(=O)C(=O)OCC.O=c1[nH]c2cc(Br)ccc2c(=O)o1
CCOC(=O)c1nc2cc(Br)ccc2c(O)c1C(=O)OCC
null
null
CN(C=O)C
Miscellaneous
OtherReaction
6a57a3597d32a89058ecee7d5f10c7dfe66b566f5458c9a02f9ca35e0d21a60d
9da8ba30ba25142ceb94d865cd4c0f29929d07b92e6a842861f67100ed84de1c
c1ccc2ncccc2c1
O=[C;H0;D3;+0:1](-[CH2;D2;+0:2]-[C:3](=[O;D1;H0:4])-[#8:5]-[C:6])-[C:7](=[O;D1;H0:8])-[#8:9]-[C:10].O=[c;H0;D3;+0:11]1:[o;H0;D2;+0:12]:c(=O):[nH;D2;+0:13]:[c:14](:[c:15]):[c:16]:1:[c:17]>>[C:10]-[#8:9]-[C:7](=[O;D1;H0:8])-[c;H0;D3;+0:1]1:[c;H0;D3;+0:11](-[OH;D1;+0:12]):[c:16](:[c:17]):[c:14](:[c:15]):[n;H0;D2;+0:13]:[c...
24
[{"value": 24.0, "product": "BrC1=CC=C2C(=C(C(=NC2=C1)C(=O)OCC)C(=O)OCC)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 23.7, "product": "BrC1=CC=C2C(=C(C(=NC2=C1)C(=O)OCC)C(=O)OCC)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
130
CELSIUS
null
null
To a stirred mixture of diethyl oxosuccinate sodium salt (1.31 g, 6.23 mM) in dimethylformamide (DMF, 15 mL) under a nitrogen atmosphere was added a solution of 7-bromo-2H-3,1-benzoxazine-2,4(1H)-dione (1.50 g, 6.20 mM) in DMF (15 mL). The resulting reaction mixture was heated to 130° C. over 2.5 hr and then refluxed f...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ester.Ester
Ester.Ester.Aromatic alcohol
c1ccc2cocnc2c1
c1ccc2ncccc2c1
c1ccc2ncccc2c1
HO-
CN(C=O)C
130
null
CCOC(=O)CC(=O)C(=O)OCC.O=c1[nH]c2cc(Br)ccc2c(=O)o1>CN(C=O)C>CCOC(=O)c1nc2cc(Br)ccc2c(O)c1C(=O)OCC
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-4afa85f5bd694c988e0706bc73077ac1
O=C(Cl)CCc1ccccc1.O=c1[nH][nH]c(=O)c2c(O)c3ccc(Cl)cc3nc12>>O=C(CCc1ccccc1)Oc1n[nH]c(=O)c2nc3cc(Cl)ccc3c(O)c12
ClC=1C=CC=2C(=C3C(=NC2C1)C(NNC3=O)=O)O.C(CCC1=CC=CC=C1)(=O)Cl>>ClC=1C=CC=2C(=C3C(=NC2C1)C(NN=C3OC(CCC3=CC=CC=C3)=O)=O)O
Cl[C:2](=[O:1])[CH2:3][CH2:4][c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1.[O:11]=[c:12]1[nH:13][nH:14][c:15](=[O:16])[c:17]2[n:18][c:19]3[cH:20][c:21]([Cl:22])[cH:23][cH:24][c:25]3[c:26]([OH:27])[c:28]12>>[O:1]=[C:2]([CH2:3][CH2:4][c:5]1[cH:6][cH:7][cH:8][cH:9][cH:10]1)[O:11][c:12]1[n:13][nH:14][c:15](=[O:16])[c:17]2[n:18][c...
O=C(Cl)CCc1ccccc1.O=c1[nH][nH]c(=O)c2c(O)c3ccc(Cl)cc3nc12
O=C(CCc1ccccc1)Oc1n[nH]c(=O)c2nc3cc(Cl)ccc3c(O)c12
null
null
N1=CC=CC=C1.O
Acylation
OtherReaction
b18d846ff0412004ceb2ba9c6d237268ee56f1c008c4c07cdd457eed44dc75b6
74160603d2471b6dce676fdb61c753a80de32635d34da1c285b2b50abd3324f9
O=C(CCc1ccccc1)Oc1n[nH]c(=O)c2nc3ccccc3cc12
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]-[C:4].[O;H0;D1;+0:5]=[c;H0;D3;+0:6]1:[nH;D2;+0:7]:[#7;a:8]:[c:9]:[c:10](:[#7;a:11]:[c:12]):[c:13]:1:[c:14]>>[C:4]-[C:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[O;H0;D2;+0:5]-[c;H0;D3;+0:6]1:[n;H0;D2;+0:7]:[#7;a:8]:[c:9]:[c:10](:[#7;a:11]:[c:12]):[c:13]:1:[c:14]
null
[]
null
null
2
HOUR
A mixture of 7-chloro-2,3-dihydro-10-hydroxypyridazino[4,5-b]quinoline-1,4-dione (0.60 g, 2.3 mM), as prepared in Example 2, and hydrocinnamoyl chloride (1.15 g, 6.84 mM) in pyridine (9 mL) was refluxed for 1 hr. Upon cooling to room temperature, the solution solidified. After 2 hr at room temperature, the mixture was ...
10.6084/m9.figshare.5104873.v1
null
Acyl halide
Ester
C1=c2cc3ccccc3nc2=CNN1
c1ccc2cc3cnncc3nc2c1
c1ccccc1.c1ccc2cc3cnncc3nc2c1
HCl
N1=CC=CC=C1.O
null
2
O=C(Cl)CCc1ccccc1.O=c1[nH][nH]c(=O)c2c(O)c3ccc(Cl)cc3nc12>N1=CC=CC=C1.O>O=C(CCc1ccccc1)Oc1n[nH]c(=O)c2nc3cc(Cl)ccc3c(O)c12
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-dd94778e10ec4f848d748b205dfbec9e
CCOC(=O)CC(=O)C(=O)OCC.O=c1[nH]c2c(Cl)cccc2c(=O)o1>>CCOC(=O)c1nc2c(Cl)cccc2c(O)c1C(=O)OCC
[Na].O=C(C(=O)OCC)CC(=O)OCC.ClC1=CC=CC=2C(OC(NC21)=O)=O.O>>ClC=1C=CC=C2C(=C(C(=NC12)C(=O)OCC)C(=O)OCC)O
O=[C:17]([CH2:6][C:4]([O:3][CH2:2][CH3:1])=[O:5])[C:18](=[O:19])[O:20][CH2:21][CH3:22].O=c1[nH:7][c:8]2[c:9]([Cl:10])[cH:11][cH:12][cH:13][c:14]2[c:15](=O)[o:16]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[n:7][c:8]2[c:9]([Cl:10])[cH:11][cH:12][cH:13][c:14]2[c:15]([OH:16])[c:17]1[C:18](=[O:19])[O:20][CH2:21][CH3:22]
CCOC(=O)CC(=O)C(=O)OCC.O=c1[nH]c2c(Cl)cccc2c(=O)o1
CCOC(=O)c1nc2c(Cl)cccc2c(O)c1C(=O)OCC
null
null
CN(C=O)C
Miscellaneous
OtherReaction
2eef483005397da632942cbbc21d7e5da2fabb0c9f19f10dc593f88983716aee
9da8ba30ba25142ceb94d865cd4c0f29929d07b92e6a842861f67100ed84de1c
c1ccc2ncccc2c1
O=[C;H0;D3;+0:1](-[CH2;D2;+0:2]-[C:3](=[O;D1;H0:4])-[#8:5]-[C:6])-[C:7](=[O;D1;H0:8])-[#8:9]-[C:10].O=[c;H0;D3;+0:11]1:[o;H0;D2;+0:12]:c(=O):[nH;D2;+0:13]:[c:14](:[c:15]):[c:16]:1:[c:17]>>[C:10]-[#8:9]-[C:7](=[O;D1;H0:8])-[c;H0;D3;+0:1]1:[c;H0;D3;+0:11](-[OH;D1;+0:12]):[c:16](:[c:17]):[c:14](:[c:15]):[n;H0;D2;+0:13]:[c...
43.8
[{"value": 43.8, "product": "ClC=1C=CC=C2C(=C(C(=NC12)C(=O)OCC)C(=O)OCC)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
130
CELSIUS
null
null
To a stirred mixture of diethyl oxosuccinate sodium salt (2.31 g, 11.0 mM) in dimethylformamide (20 mL) under a nitrogen atmosphere was added 8-chloro-2H-3,1-benzoxazine-2,4(1H)-dione (2.17 g, 11.0 mM). The resulting mixture was heated slowly to 130° C. and maintained at this temperature for 2.5 hr. After cooling, the ...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ester.Ester
Ester.Ester.Aromatic alcohol
c1ocnc2ccccc12
c1ccc2ncccc2c1
c1ccc2ncccc2c1
HO-
CN(C=O)C
130
null
CCOC(=O)CC(=O)C(=O)OCC.O=c1[nH]c2c(Cl)cccc2c(=O)o1>CN(C=O)C>CCOC(=O)c1nc2c(Cl)cccc2c(O)c1C(=O)OCC
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-b6d9760dfaec4627a210e1ab02e7806c
O=c1[nH]c2cccc(I)c2c(=O)o1>>COC(=O)c1c(N)cccc1I
[OH-].[Na+].IC1=CC=CC2=C1C(OC(N2)=O)=O>>NC1=C(C(=O)OC)C(=CC=C1)I
O=[c:1]1[o:2][c:3](=[O:4])[c:5]2[c:6]([nH:7]1)[cH:8][cH:9][cH:10][c:11]2[I:12]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[c:6]([NH2:7])[cH:8][cH:9][cH:10][c:11]1[I:12]
O=c1[nH]c2cccc(I)c2c(=O)o1
COC(=O)c1c(N)cccc1I
null
[OH-].[Na+]
CO
Reduction
OtherReaction
4a877ce7f9d8b0e05ec6ae8c859c09c08e7f1fd55a56b7ca38718591b6593140
9f87be38aa9793f80b3cef223629015a04ccba30a9633b313486e0a6edc9c43d
c1ccccc1
O=[c;H0;D3;+0:1]1:[nH;D2;+0:2]:[c:3](:[c:4]):[c:5](:[c:6]):[c;H0;D3;+0:7](=[O;D1;H0:8]):[o;H0;D2;+0:9]:1>>[CH3;D1;+0:1]-[O;H0;D2;+0:9]-[C;H0;D3;+0:7](=[O;D1;H0:8])-[c:5](:[c:6]):[c:3](-[NH2;D1;+0:2]):[c:4]
78.4
[{"value": 78.4, "product": "NC1=C(C(=O)OC)C(=CC=C1)I", "details": "PERCENTYIELD", "is_desired": false}, {"value": 78.4, "product": "NC1=C(C(=O)OC)C(=CC=C1)I", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
1
HOUR
To a stirred solution of sodium hydroxide (0.35 g, 8.8 mM) in methanol (31 mL) was added 5-iodo-2H-3,1-benzoxazine-2,4(1H)-dione (18.5 g, 64.0 mM). The mixture was heated at 60° C. for 1.5 hr. An additional quantitiy of sodium hydroxide (0.10 g, 2.5 mM) was added to the reaction mixture and stirring at 60° C. was conti...
10.6084/m9.figshare.5104873.v1
null
null
Ester.Primary amine
c1nc2ccccc2co1
c1ccccc1
c1ccccc1
Other
[OH-].[Na+].CO
60
1
O=c1[nH]c2cccc(I)c2c(=O)o1>[OH-].[Na+].CO>COC(=O)c1c(N)cccc1I
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-d1949a80f5a34ab9a1a505ee7b40c299
COc1c(Cl)cc([N+](=O)[O-])cc1Cl>>COc1c(Cl)cc(N)cc1Cl
[OH-].[Na+].ClC1=C(C(=CC(=C1)[N+](=O)[O-])Cl)OC.O.O.[Sn](Cl)Cl>>ClC=1C=C(N)C=C(C1OC)Cl
O=[N+:8]([O-])[c:7]1[cH:6][c:4]([Cl:5])[c:3]([O:2][CH3:1])[c:10]([Cl:11])[cH:9]1>>[CH3:1][O:2][c:3]1[c:4]([Cl:5])[cH:6][c:7]([NH2:8])[cH:9][c:10]1[Cl:11]
COc1c(Cl)cc([N+](=O)[O-])cc1Cl
COc1c(Cl)cc(N)cc1Cl
null
null
C(C)O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccccc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
83.7
[{"value": 83.7, "product": "ClC=1C=C(N)C=C(C1OC)Cl", "details": "PERCENTYIELD", "is_desired": false}, {"value": 83.7, "product": "ClC=1C=C(N)C=C(C1OC)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A stirred mixture of 2,6-dichloro-4-nitroanisole (4.6 g, 21 mM) and tin(II) dichloride dihydrate (23.4 g, 104 mM) in ethanol (72 mL) was refluxed for 3 hr. After cooling to room temperature, the reaction mixture was poured into ice water which was then treated with 2N sodium hydroxide until the solution became basic. T...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1
Other
C(C)O
null
null
COc1c(Cl)cc([N+](=O)[O-])cc1Cl>C(C)O>COc1c(Cl)cc(N)cc1Cl
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-96c9427d56a846deb08ae5a7e598c8e7
CI.COc1c(Cl)cc(NC(=O)OC(C)(C)C)c(C(=O)O)c1Cl>>COC(=O)c1c(NC(=O)OC(C)(C)C)cc(Cl)c(OC)c1Cl
O.[H-].[Na+].C(C)(C)(C)OC(=O)NC1=C(C(=O)O)C(=C(C(=C1)Cl)OC)Cl.IC>>C(C)(C)(C)OC(=O)NC1=C(C(=O)OC)C(=C(C(=C1)Cl)OC)Cl
I[CH3:1].[OH:2][C:3](=[O:4])[c:5]1[c:6]([NH:7][C:8](=[O:9])[O:10][C:11]([CH3:12])([CH3:13])[CH3:14])[cH:15][c:16]([Cl:17])[c:18]([O:19][CH3:20])[c:21]1[Cl:22]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[c:6]([NH:7][C:8](=[O:9])[O:10][C:11]([CH3:12])([CH3:13])[CH3:14])[cH:15][c:16]([Cl:17])[c:18]([O:19][CH3:20])[c:21]1[Cl:22]
CI.COc1c(Cl)cc(NC(=O)OC(C)(C)C)c(C(=O)O)c1Cl
COC(=O)c1c(NC(=O)OC(C)(C)C)cc(Cl)c(OC)c1Cl
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
9474aa79a2adc7353c0c02444ca598a6f486ecdd7ed5edb9ae0645721ee50389
badd4f82161bb0ee7acffd023ea4caae5d036bce7065c10ab0a06e83a6a6f119
c1ccccc1
I-[CH3;D1;+0:1].[O;D1;H0:2]=[C:3](-[OH;D1;+0:4])-[c:5]>>[CH3;D1;+0:1]-[O;H0;D2;+0:4]-[C:3](=[O;D1;H0:2])-[c:5]
96
[{"value": 96.0, "product": "C(C)(C)(C)OC(=O)NC1=C(C(=O)OC)C(=C(C(=C1)Cl)OC)Cl", "details": "PERCENTYIELD", "is_desired": false}, {"value": 96.0, "product": "C(C)(C)(C)OC(=O)NC1=C(C(=O)OC)C(=C(C(=C1)Cl)OC)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a cold (ice bath) stirred solution of 2-(tert-butoxycarbonylamino)-4,6-dichloro-5-methoxybenzoic acid (2.0 g, 5.9 mM) in 20 mL of dry dimethylformamide under a nitrogen atmosphere was added sodium hydride (0.24 g, 5.9 mM); a precipitate formed which slowly redissolved on stirring. To the resulting stirred solution w...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Ester
null
null
c1ccccc1
HI
CN(C=O)C
null
null
CI.COc1c(Cl)cc(NC(=O)OC(C)(C)C)c(C(=O)O)c1Cl>CN(C=O)C>COC(=O)c1c(NC(=O)OC(C)(C)C)cc(Cl)c(OC)c1Cl
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-8d59dafca56b4fad8c6a7600ac1e67f1
COC(=O)c1c(NC(=O)OC(C)(C)C)cc(Cl)c(OC)c1Cl>>COC(=O)c1c(N)cc(Cl)c(OC)c1Cl
C(C)(C)(C)OC(=O)NC1=C(C(=O)OC)C(=C(C(=C1)Cl)OC)Cl.FC(C(=O)O)(F)F>>NC1=C(C(=O)OC)C(=C(C(=C1)Cl)OC)Cl
CC(C)(C)OC(=O)[NH:7][c:6]1[c:5]([C:3]([O:2][CH3:1])=[O:4])[c:14]([Cl:15])[c:11]([O:12][CH3:13])[c:9]([Cl:10])[cH:8]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[c:6]([NH2:7])[cH:8][c:9]([Cl:10])[c:11]([O:12][CH3:13])[c:14]1[Cl:15]
COC(=O)c1c(NC(=O)OC(C)(C)C)cc(Cl)c(OC)c1Cl
COC(=O)c1c(N)cc(Cl)c(OC)c1Cl
null
null
C(Cl)Cl
Reduction
Hydrogenolysis of amides/imides/carbamates
3c33dd2a2d355ee5ba0287367e209aa147a39aa00607f0c95fb2bf1ade45d014
c5b5dffe7dd8beebdc1baa8b5b05300a9f7079e65dcfd42ade6f8a77ff09537d
c1ccccc1
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[c:2](:[c:3]):[c:4]-[C:5](-[#8:6])=[O;D1;H0:7]>>[#8:6]-[C:5](=[O;D1;H0:7])-[c:4]:[c:2](-[NH2;D1;+0:1]):[c:3]
87
[{"value": 87.0, "product": "NC1=C(C(=O)OC)C(=C(C(=C1)Cl)OC)Cl", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution o#methyl 2-(tert-butoxycarbonylamino)-4,6-dichloro-5-methoxybenzoate (2.3 g, 6.6 mM) and trifluoroacetic acid (6.0 g, 53 mM) in methylene chloride (23 mL) was stirred at room temperature for 1.5 hr. The reaction mixture was then washed with saturated aqueous sodium bicarbonate, drie (MgSO4), filtered and con...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Primary amine
null
null
c1ccccc1
HO-
C(Cl)Cl
null
null
COC(=O)c1c(NC(=O)OC(C)(C)C)cc(Cl)c(OC)c1Cl>C(Cl)Cl>COC(=O)c1c(N)cc(Cl)c(OC)c1Cl
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-212e81895b584e808d5abbbb91d99bed
CCc1cc(Br)cc2c1C(=O)C(=O)N2.O=C(O)c1cccc(OO)c1C(=O)O>>CCc1cc(Br)cc2[nH]c(=O)oc(=O)c12
O.BrC1=CC(=C2C(C(NC2=C1)=O)=O)CC.C1=CC(=C(C(=C1)OO)C(=O)O)C(=O)O>>BrC1=CC2=C(C(OC(N2)=O)=O)C(=C1)CC
[CH3:1][CH2:2][c:3]1[cH:4][c:5]([Br:6])[cH:7][c:8]2[c:15]1[C:13](=[O:14])[C:10](=[O:11])[NH:9]2.O=C(O)c1c(OO)cccc1C(=O)[OH:12]>>[CH3:1][CH2:2][c:3]1[cH:4][c:5]([Br:6])[cH:7][c:8]2[nH:9][c:10](=[O:11])[o:12][c:13](=[O:14])[c:15]12
CCc1cc(Br)cc2c1C(=O)C(=O)N2.O=C(O)c1cccc(OO)c1C(=O)O
CCc1cc(Br)cc2[nH]c(=O)oc(=O)c12
null
null
C(C)(=O)O
Miscellaneous
OtherReaction
c2de0b94b09bdf803797c35375a584c41aaa053492f400c41ac8174d57dd96c3
23ca1a4188e84983b2834b492c533f8abb5826e748f0ff4dba158b499183ccaa
O=c1[nH]c2ccccc2c(=O)o1
O-O-c1:c:c:c:c(-C(=O)-[OH;D1;+0:1]):c:1-C(-O)=O.[O;D1;H0:2]=[C;H0;D3;+0:3]1-[NH;D2;+0:4]-[c:5](:[c:6]):[c:7](:[c:8])-[C;H0;D3;+0:9]-1=[O;D1;H0:10]>>[O;D1;H0:2]=[c;H0;D3;+0:3]1:[nH;D2;+0:4]:[c:5](:[c:6]):[c:7](:[c:8]):[c;H0;D3;+0:9](=[O;D1;H0:10]):[o;H0;D2;+0:1]:1
null
[]
null
null
null
null
A stirred solution of 6-bromo-4-ethyl-1H-indole-2,3-dione (2.64 g, 10.4 mM) and the hexahydrate magnesium salt of monoperoxyphthalic acid (80% pure, 3.54 g, 5.73 mM) in glacial acetic acid (30 mL) was stirred at 60° C. for 1 hr during which time a precipitate formed. The cooled reaction mixture was then poured into col...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Carboxylic acid.Ketone.Secondary amide.Peroxide
null
c1ccc2c(c1)CCN2.c1ccccc1
c1ccc2cocnc2c1
c1ccc2cocnc2c1
HO-
C(C)(=O)O
null
null
CCc1cc(Br)cc2c1C(=O)C(=O)N2.O=C(O)c1cccc(OO)c1C(=O)O>C(C)(=O)O>CCc1cc(Br)cc2[nH]c(=O)oc(=O)c12
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-1eb43454a5ef481dbf4ca95331913c1b
CC(C)(C)OC(=O)Nc1cc(Cl)cc(C(F)(F)F)c1.O=C=O>>CC(C)(C)OC(=O)c1cc(C(F)(F)F)cc(Cl)c1C(=O)O
O.C(C)(C)(C)OC(=O)NC1=CC(=CC(=C1)C(F)(F)F)Cl.O1CCCC1.C(C)(C)(C)[Li].C(=O)=O>>C(C)(C)(C)OC(=O)C1=C(C(=O)O)C(=CC(=C1)C(F)(F)F)Cl
N([C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[c:8]1[cH:9][c:10]([C:11]([F:12])([F:13])[F:14])[cH:15][c:16]([Cl:17])[cH:18]1.[C:19](=[O:20])=[O:21]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[c:8]1[cH:9][c:10]([C:11]([F:12])([F:13])[F:14])[cH:15][c:16]([Cl:17])[c:18]1[C:19](=[O:20])[OH:21]
CC(C)(C)OC(=O)Nc1cc(Cl)cc(C(F)(F)F)c1.O=C=O
CC(C)(C)OC(=O)c1cc(C(F)(F)F)cc(Cl)c1C(=O)O
null
null
CCCCC
Acylation
OtherReaction
475bed91ea8d3dff3b5c1b6e17807dec7cd6c0c6ce79e792e8fab4b47f7eaa2f
210646275b30fec4c694f5e99452fb6596cdedc38c8ab4483898d142267efae2
c1ccccc1
[C;D1;H3:1]-[C:2](-[C;D1;H3:3])(-[C;D1;H3:4])-[#8:5]-[C;H0;D3;+0:6](=[O;D1;H0:7])-N-[c;H0;D3;+0:8]1:[c:9]:[c:10]:[c:11]:[c:12](-[Cl;D1;H0:13]):[cH;D2;+0:14]:1.[O;D1;H0:15]=[C;H0;D2;+0:16]=[O;H0;D1;+0:17]>>[C;D1;H3:1]-[C:2](-[C;D1;H3:3])(-[C;D1;H3:4])-[#8:5]-[C;H0;D3;+0:6](=[O;D1;H0:7])-[c;H0;D3;+0:8]1:[c:9]:[c:10]:[c:1...
82
[{"value": 82.0, "product": "C(C)(C)(C)OC(=O)C1=C(C(=O)O)C(=CC(=C1)C(F)(F)F)Cl", "details": "PERCENTYIELD", "is_desired": false}]
-75
CELSIUS
null
null
To a cold (-100° C.) stirred solution of N-(tert-butoxycarbonyl)-3-chloro-5-trifluoromethylaniline 93.4 g, 11.5 mM) in dry tetrahydrofuran (30 mL) under a nitrogen atmosphere was added dropwise t-butyllithium (14.2 mL of 1.7 M solution, 24.2 mM) in pentane. The temperature of the reaction mixture was maintained at -103...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Carbon dioxide.Boc
Carboxylic acid.Ester.Boc
c1ccccc1
c1ccccc1
c1ccccc1
Other
CCCCC
-75
null
CC(C)(C)OC(=O)Nc1cc(Cl)cc(C(F)(F)F)c1.O=C=O>CCCCC>CC(C)(C)OC(=O)c1cc(C(F)(F)F)cc(Cl)c1C(=O)O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-0600c001c51645919f6df926c38c5514
Nc1cc(Cl)cc(C(F)(F)F)c1C(=O)O.O=C(OC(Cl)(Cl)Cl)OC(Cl)(Cl)Cl>>O=c1[nH]c2cc(C(F)(F)F)cc(Cl)c2c(=O)o1
O.NC1=C(C(=O)O)C(=CC(=C1)Cl)C(F)(F)F.ClC(Cl)(Cl)OC(OC(Cl)(Cl)Cl)=O>>ClC1=CC(=CC2=C1C(OC(N2)=O)=O)C(F)(F)F
[NH2:3][c:4]1[cH:5][c:12]([Cl:13])[cH:11][c:6]([C:7]([F:8])([F:9])[F:10])[c:14]1[C:15](=[O:16])[OH:17].ClC(Cl)(Cl)O[C:2](OC(Cl)(Cl)Cl)=[O:1]>>[O:1]=[c:2]1[nH:3][c:4]2[cH:5][c:6]([C:7]([F:8])([F:9])[F:10])[cH:11][c:12]([Cl:13])[c:14]2[c:15](=[O:16])[o:17]1
Nc1cc(Cl)cc(C(F)(F)F)c1C(=O)O.O=C(OC(Cl)(Cl)Cl)OC(Cl)(Cl)Cl
O=c1[nH]c2cc(C(F)(F)F)cc(Cl)c2c(=O)o1
null
null
O1CCCC1
Aromatic Heterocycle Formation
OtherReaction
473d8917d142d976b6bbb3c47c54cadfe4d17a751eabb736fd7b01b50c3ead61
8337e7dcd80ae495bd7effbccbb483dc6496434024ea4407e426959abd54f128
O=c1[nH]c2ccccc2c(=O)o1
Cl-C(-Cl)(-Cl)-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-O-C(-Cl)(-Cl)-Cl.[Cl;D1;H0:3]-[c;H0;D3;+0:4]1:[c:5]:[c;H0;D3;+0:6](-[C:7](-[F;D1;H0:8])(-[F;D1;H0:9])-[F;D1;H0:10]):[c;H0;D3;+0:11](-[C;H0;D3;+0:12](=[O;D1;H0:13])-[OH;D1;+0:14]):[c:15](-[NH2;D1;+0:16]):[cH;D2;+0:17]:1>>[Cl;D1;H0:3]-[c;H0;D3;+0:4]1:[c:5]:[c;H0;D3;+0:6](-[C:...
null
[]
null
null
2
HOUR
To a stirred solution of 2-amino-4-chloro-6-trifluoromethylbenzoic acid (0.53 g, 2.2 mM) in dry tetrahydrofuran (6 mL) under a nitrogen atmosphere was added bis(trichloromethyl)carbonate (0.218 g, 0.734 mM). The resulting solution was stirred at room temperature for 2 hr, poured into water and the resulting mixture ext...
10.6084/m9.figshare.5104873.v1
null
Trichloro group.Trichloro group.Aromatic halide.Carbonic Ester.Carboxylic acid.Primary amine
Aromatic halide
c1ccccc1
c1ccc2cocnc2c1
c1ccc2cocnc2c1
HCl
O1CCCC1
null
2
Nc1cc(Cl)cc(C(F)(F)F)c1C(=O)O.O=C(OC(Cl)(Cl)Cl)OC(Cl)(Cl)Cl>O1CCCC1>O=c1[nH]c2cc(C(F)(F)F)cc(Cl)c2c(=O)o1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-de691adb4df542928566b3b06e2c218d
O=c1[nH]c2cc(C(F)(F)F)cc(Cl)c2c(=O)o1>>COC(=O)c1c(N)cc(C(F)(F)F)cc1Cl
C(C)OCC.[OH-].[Na+].ClC1=CC(=CC2=C1C(OC(N2)=O)=O)C(F)(F)F>>NC1=C(C(=O)OC)C(=CC(=C1)C(F)(F)F)Cl
O=[c:1]1[o:2][c:3](=[O:4])[c:5]2[c:6]([nH:7]1)[cH:8][c:9]([C:10]([F:11])([F:12])[F:13])[cH:14][c:15]2[Cl:16]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[c:6]([NH2:7])[cH:8][c:9]([C:10]([F:11])([F:12])[F:13])[cH:14][c:15]1[Cl:16]
O=c1[nH]c2cc(C(F)(F)F)cc(Cl)c2c(=O)o1
COC(=O)c1c(N)cc(C(F)(F)F)cc1Cl
null
null
CO
Reduction
OtherReaction
fb3a8999d982d1c42a150fbbeb96fa0db2838a9c48a5140f183de4d3421c8ad6
9f87be38aa9793f80b3cef223629015a04ccba30a9633b313486e0a6edc9c43d
c1ccccc1
O=[c;H0;D3;+0:1]1:[nH;D2;+0:2]:[c:3](:[c:4]):[c:5](:[c:6]):[c;H0;D3;+0:7](=[O;D1;H0:8]):[o;H0;D2;+0:9]:1>>[CH3;D1;+0:1]-[O;H0;D2;+0:9]-[C;H0;D3;+0:7](=[O;D1;H0:8])-[c:5](:[c:6]):[c:3](-[NH2;D1;+0:2]):[c:4]
88
[{"value": 88.0, "product": "NC1=C(C(=O)OC)C(=CC(=C1)C(F)(F)F)Cl", "details": "PERCENTYIELD", "is_desired": false}, {"value": 87.3, "product": "NC1=C(C(=O)OC)C(=CC(=C1)C(F)(F)F)Cl", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
null
null
To a stirred solution of sodium hydroxide (0.012 g, 0.31 mM) in anhydrous methanol (1.5 mL) under a nitrogen atmosphere was added 5-chloro-7-trifluoromethyl-2H-3,1-benzoxazine-2,4(1H)-dione (0.60 g, 2.3 mM). The resulting mixture was warmed to 60° C. for 0.5 hr, allowed to cool to room temperature and poured into dieth...
10.6084/m9.figshare.5104873.v1
null
null
Ester.Primary amine
c1ccc2cocnc2c1
c1ccccc1
c1ccccc1
Other
CO
60
null
O=c1[nH]c2cc(C(F)(F)F)cc(Cl)c2c(=O)o1>CO>COC(=O)c1c(N)cc(C(F)(F)F)cc1Cl
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-fb1f425ed29c488e8ffdf69649ec7433
Nc1cc(F)ccc1C(=O)O>>COC(=O)c1ccc(F)cc1N
C([O-])(O)=O.[Na+].NC1=C(C(=O)O)C=CC(=C1)F.Cl.Cl>>NC1=C(C(=O)OC)C=CC(=C1)F
[OH:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([F:9])[cH:10][c:11]1[NH2:12]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([F:9])[cH:10][c:11]1[NH2:12]
Nc1cc(F)ccc1C(=O)O
COC(=O)c1ccc(F)cc1N
null
null
CO.O
Miscellaneous
Protection of carboxylic acid
56520e0abb4535dce9a663824ca803b71c2c0dd72dfd246317d953596a987bd2
2ccc7a30191c2c171b49e8a0217bee87430687dd0f567141eca025a75b7e3136
c1ccccc1
[O;D1;H0:1]=[C:2](-[OH;D1;+0:3])-[c:4]>>[C;D1;H3:5]-[O;H0;D2;+0:3]-[C:2](=[O;D1;H0:1])-[c:4]
80.6
[{"value": 80.6, "product": "NC1=C(C(=O)OC)C=CC(=C1)F", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A stirred solution of 2-amino-4-fluorobenzoic acid (4.86 g, 31.3 mM) in anhydrous methanol (100 mL) was saturated with anhydrous hydrogen chloride and then refluxed for 4 days. During the reflux period, the reaction mixture was periodically resaturated with hydrogen chloride. After the reflux period, the reaction mixtu...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Ester
null
null
c1ccccc1
Other
CO.O
null
null
Nc1cc(F)ccc1C(=O)O>CO.O>COC(=O)c1ccc(F)cc1N
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-d22c33b8f7f941c2ae9d370668c316af
CCOC(=O)c1nc2ccc([N+](=O)[O-])cc2c(O)c1C(=O)OCC>>CCOC(=O)c1nc2ccc(N)cc2c(O)c1C(=O)OCC
OC1=C(C(=NC2=CC=C(C=C12)[N+](=O)[O-])C(=O)OCC)C(=O)OCC.C(C)(=O)O>>NC=1C=C2C(=C(C(=NC2=CC1)C(=O)OCC)C(=O)OCC)O
O=[N+:12]([O-])[c:11]1[cH:10][cH:9][c:8]2[n:7][c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[c:17]([C:18](=[O:19])[O:20][CH2:21][CH3:22])[c:15]([OH:16])[c:14]2[cH:13]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[n:7][c:8]2[cH:9][cH:10][c:11]([NH2:12])[cH:13][c:14]2[c:15]([OH:16])[c:17]1[C:18](=[O:19])[O:20][CH2:21][CH3:22]
CCOC(=O)c1nc2ccc([N+](=O)[O-])cc2c(O)c1C(=O)OCC
CCOC(=O)c1nc2ccc(N)cc2c(O)c1C(=O)OCC
null
[Fe]
C(C)O
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccc2ncccc2c1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
75.3
[{"value": 75.3, "product": "NC=1C=C2C(=C(C(=NC2=CC1)C(=O)OCC)C(=O)OCC)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 75.1, "product": "NC=1C=C2C(=C(C(=NC2=CC1)C(=O)OCC)C(=O)OCC)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A stirred mixture of diethyl 4-hydroxy-6-nitroquinoline-2,3-dicarboxylate (4.4 g, 13 mM), powdered iron (6.6 g, 118 mM) and glacial acetic acid (18.5 g, 307 mM) in ethanol (80 mL) was refluxed for 20 hr under a nitrogen atmosphere. The reaction mixture was cooled and filtered and the filtrate was concentrated. The dark...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccc2ncccc2c1
Other
[Fe].C(C)O
null
null
CCOC(=O)c1nc2ccc([N+](=O)[O-])cc2c(O)c1C(=O)OCC>[Fe].C(C)O>CCOC(=O)c1nc2ccc(N)cc2c(O)c1C(=O)OCC
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-b9d0a22ff2cb4115aad368a06d554f16
CCc1cc(Br)c2c(O)c(C(=O)NN)c(C(=O)NN)nc2c1>>CCc1cc(Br)c2c(O)c3c(=O)[nH][nH]c(=O)c3nc2c1
N(N)C(=O)C1=NC2=CC(=CC(=C2C(=C1C(=O)NN)O)Br)CC>>BrC=1C=2C(=C3C(=NC2C=C(C1)CC)C(NNC3=O)=O)O
NN[C:15](=[O:16])[c:17]1[c:10]([C:11](=[O:12])[NH:13][NH2:14])[c:8]([OH:9])[c:7]2[c:5]([Br:6])[cH:4][c:3]([CH2:2][CH3:1])[cH:20][c:19]2[n:18]1>>[CH3:1][CH2:2][c:3]1[cH:4][c:5]([Br:6])[c:7]2[c:8]([OH:9])[c:10]3[c:11](=[O:12])[nH:13][nH:14][c:15](=[O:16])[c:17]3[n:18][c:19]2[cH:20]1
CCc1cc(Br)c2c(O)c(C(=O)NN)c(C(=O)NN)nc2c1
CCc1cc(Br)c2c(O)c3c(=O)[nH][nH]c(=O)c3nc2c1
null
null
C(C)(=O)O
Aromatic Heterocycle Formation
OtherReaction
f3dbb0a7ecffef3e204ef147736503e670fedb65b98cbf3d826138146a8353d2
b3d4fa0dcfa02ac7642075a89f830594ba71dc7452e661900a986719bd6ddb0a
O=c1[nH][nH]c(=O)c2nc3ccccc3cc12
N-N-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[#7;a:4]:[c:5]):[c:6](-[C;H0;D3;+0:7](=[O;D1;H0:8])-[NH;D2;+0:9]-[NH2;D1;+0:10]):[c:11]>>[O;D1;H0:8]=[c;H0;D3;+0:7]1:[nH;D2;+0:9]:[nH;D2;+0:10]:[c;H0;D3;+0:1](=[O;D1;H0:2]):[c:3](:[#7;a:4]:[c:5]):[c:6]:1:[c:11]
70
[{"value": 70.0, "product": "BrC=1C=2C(=C3C(=NC2C=C(C1)CC)C(NNC3=O)=O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 68.5, "product": "BrC=1C=2C(=C3C(=NC2C=C(C1)CC)C(NNC3=O)=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
81
CELSIUS
null
null
A stirred mixture of 2,3-bishydrazinocarbonyl-5-bromo-7-ethyl-4-hydroxyquinoline (0.40 g, 1.1 mM) in glacial acetic acid (12 mL) was heated at 81° C. for 1.5 hr. After cooling to room temperature, the reaction mixture was filtered and the collected solids washed with acetic acid and air dried to provide the title compo...
10.6084/m9.figshare.5104873.v1
null
Acylhydrazine.Acylhydrazine
null
c1ccc2ncccc2c1
C1=c2cc3ccccc3nc2=CNN1
C1=c2cc3ccccc3nc2=CNN1
Other
C(C)(=O)O
81
null
CCc1cc(Br)c2c(O)c(C(=O)NN)c(C(=O)NN)nc2c1>C(C)(=O)O>CCc1cc(Br)c2c(O)c3c(=O)[nH][nH]c(=O)c3nc2c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-29cf4cf9cdd54ff580a9152a0791fb0b
Cc1ccc(N)c([N+](=O)[O-])c1.ClCl>>Cc1cc(Cl)c(N)c([N+](=O)[O-])c1
CC1=CC(=C(N)C=C1)[N+](=O)[O-].ClCl>>ClC1=C(N)C(=CC(=C1)C)[N+](=O)[O-]
[CH3:1][c:2]1[cH:3][cH:4][c:6]([NH2:7])[c:8]([N+:9](=[O:10])[O-:11])[cH:12]1.Cl[Cl:5]>>[CH3:1][c:2]1[cH:3][c:4]([Cl:5])[c:6]([NH2:7])[c:8]([N+:9](=[O:10])[O-:11])[cH:12]1
Cc1ccc(N)c([N+](=O)[O-])c1.ClCl
Cc1cc(Cl)c(N)c([N+](=O)[O-])c1
null
null
C(Cl)(Cl)Cl
Functional Group Interconversion
Chlorination
f6effe61353895b318215d8bd9b6bb1105cafbf7be8c217d748df587260b32c3
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
c1ccccc1
Cl-[Cl;H0;D1;+0:1].[N;D1;H2:2]-[c:3](:[c:4]):[cH;D2;+0:5]:[c:6]:[c:7]>>[Cl;H0;D1;+0:1]-[c;H0;D3;+0:5](:[c:6]:[c:7]):[c:3](-[N;D1;H2:2]):[c:4]
25
[{"value": 25.0, "product": "ClC1=C(N)C(=CC(=C1)C)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 25.0, "product": "ClC1=C(N)C(=CC(=C1)C)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
DAY
To a stirred solution of 4-methyl-2-nitroaniline (19.69 g, 129.4 mM) in chloroform (200 mL) under a nitrogen atmosphere was added dropwise a solution of chlorine (10.15 g, 285.9 mM) in chloroform (100 mL) while maintaining the reaction mixture temperature below 30° C. The reaction mixture was stirred for 3 days and the...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccccc1
c1ccccc1
c1ccccc1
HCl
C(Cl)(Cl)Cl
null
72
Cc1ccc(N)c([N+](=O)[O-])c1.ClCl>C(Cl)(Cl)Cl>Cc1cc(Cl)c(N)c([N+](=O)[O-])c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-b5beb2924d104c099a4a39902f3b9c14
Cc1cc(Cl)c(N)c([N+](=O)[O-])c1>>Cc1cc(Cl)cc([N+](=O)[O-])c1
N(=O)[O-].[Na+].ClC1=C(N)C(=CC(=C1)C)[N+](=O)[O-].S(O)(O)(=O)=O>>ClC=1C=C(C=C(C1)[N+](=O)[O-])C
N[c:6]1[c:4]([Cl:5])[cH:3][c:2]([CH3:1])[cH:11][c:7]1[N+:8](=[O:9])[O-:10]>>[CH3:1][c:2]1[cH:3][c:4]([Cl:5])[cH:6][c:7]([N+:8](=[O:9])[O-:10])[cH:11]1
Cc1cc(Cl)c(N)c([N+](=O)[O-])c1
Cc1cc(Cl)cc([N+](=O)[O-])c1
null
null
C(C)O.O
Reduction
OtherReaction
a069304de6b46c6d557b2e80c544464adc3bb98001f26c098e87c25f29d552f9
a4f16f822d2806606c05d0c4baa1761ad37a11006840dde863a01a253bdff5dd
c1ccccc1
N-[c;H0;D3;+0:1](:[c:2](-[Cl;D1;H0:3]):[c:4]):[c:5](-[#7;+:6]):[c:7]>>[#7;+:6]-[c:5](:[c:7]):[cH;D2;+0:1]:[c:2](-[Cl;D1;H0:3]):[c:4]
92
[{"value": 92.0, "product": "ClC=1C=C(C=C(C1)[N+](=O)[O-])C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 92.0, "product": "ClC=1C=C(C=C(C1)[N+](=O)[O-])C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
0.5
HOUR
To a stirred mixture of 2-chloro-4-methyl-6-nitroaniline (7.39 g, 39.7 mM) and concentrated sulfuric acid (6.2 mL) in absolute ethanol (50 mL) at 0°-5° C. was slowly added a solution of sodium nitrite (6.85 g, 99.3 mM) in water (6 mL). The temperature of the reaction mixture was not allowed to exceed 5° C. during the a...
10.6084/m9.figshare.5104873.v1
null
Primary amine
null
c1ccccc1
c1ccccc1
c1ccccc1
Other
C(C)O.O
null
0.5
Cc1cc(Cl)c(N)c([N+](=O)[O-])c1>C(C)O.O>Cc1cc(Cl)cc([N+](=O)[O-])c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-4061f90aaff7419f9113b9addf8ac370
O=c1[nH][nH]c(=O)c2c(O)c3ccc(Cl)cc3nc12>>O=c1[nH][nH]c(=O)c2c(O)c3ccc(Cl)cc3nc12
CO.[OH-].OCC[N+](C)(C)C.ClC=1C=CC=2C(=C3C(=NC2C1)C(NNC3=O)=O)O.C1(=CC=CC=C1)C>>OCC[N+](C)(C)C.ClC=1C=CC=2C(=C3C(=NC2C1)C(NNC3=O)=O)O
[O:8]=[c:9]1[nH:10][nH:11][c:12](=[O:13])[c:14]2[c:15]([OH:16])[c:17]3[cH:18][cH:19][c:20]([Cl:21])[cH:22][c:23]3[n:24][c:25]12>>[O:8]=[c:9]1[nH:10][nH:11][c:12](=[O:13])[c:14]2[c:15]([OH:16])[c:17]3[cH:18][cH:19][c:20]([Cl:21])[cH:22][c:23]3[n:24][c:25]12
O=c1[nH][nH]c(=O)c2c(O)c3ccc(Cl)cc3nc12
O=c1[nH][nH]c(=O)c2c(O)c3ccc(Cl)cc3nc12
null
null
O
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
O=c1[nH][nH]c(=O)c2nc3ccccc3cc12
null
55
[{"value": 55.0, "product": "OCC[N+](C)(C)C.ClC=1C=CC=2C(=C3C(=NC2C1)C(NNC3=O)=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
To a stirred suspension of 7-chloro-2,3-dihydro-10-hydroxypyridazino[4,5-b]quinoline-1,4-dione (1.00 g, 3.8 mM) in water (40 mL) was added choline hydroxide (0.86 mL, 3.8 mM, 50 weight per cent, aqueous solution). Toluene (250 mL) was added to the resulting solution and the mixture was concentrated using a rotary evapo...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
C1=c2cc3ccccc3nc2=CNN1
null
O
null
null
O=c1[nH][nH]c(=O)c2c(O)c3ccc(Cl)cc3nc12>O>O=c1[nH][nH]c(=O)c2c(O)c3ccc(Cl)cc3nc12
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-0d0496f4365345e6a41504bd3b92e14d
CCOC(=O)CCNc1c2ccc(Cl)cc2nc2c(=O)[nH][nH]c(=O)c12>>O=C(O)CCNc1c2ccc(Cl)cc2nc2c(=O)[nH][nH]c(=O)c12
C(C)OC(=O)CCNC1=C2C(=NC=3C=C(C=CC13)Cl)C(NNC2=O)=O.Cl>>C(=O)(O)CCNC1=C2C(=NC=3C=C(C=CC13)Cl)C(NNC2=O)=O
CC[O:3][C:2](=[O:1])[CH2:4][CH2:5][NH:6][c:7]1[c:8]2[cH:9][cH:10][c:11]([Cl:12])[cH:13][c:14]2[n:15][c:16]2[c:17](=[O:18])[nH:19][nH:20][c:21](=[O:22])[c:23]12>>[O:1]=[C:2]([OH:3])[CH2:4][CH2:5][NH:6][c:7]1[c:8]2[cH:9][cH:10][c:11]([Cl:12])[cH:13][c:14]2[n:15][c:16]2[c:17](=[O:18])[nH:19][nH:20][c:21](=[O:22])[c:23]12
CCOC(=O)CCNc1c2ccc(Cl)cc2nc2c(=O)[nH][nH]c(=O)c12
O=C(O)CCNc1c2ccc(Cl)cc2nc2c(=O)[nH][nH]c(=O)c12
null
null
null
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=c1[nH][nH]c(=O)c2nc3ccccc3cc12
C-C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
97
[{"value": 97.0, "product": "C(=O)(O)CCNC1=C2C(=NC=3C=C(C=CC13)Cl)C(NNC2=O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 94.8, "product": "C(=O)(O)CCNC1=C2C(=NC=3C=C(C=CC13)Cl)C(NNC2=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 10-(2-ethoxycarbonylethylamino)-7-chloro-2,3-dihydropyridazino[4,5-b]quinoline-1,4-dione (0.08 g, 0.22 mM) and 1N hydrochloric acid was refluxed for 1 hr and then cooled to room temperature and filtered. The collected orange solid was washed with water and air dried to provide (0.07 g, 97%) the title compo...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
C1=c2cc3ccccc3nc2=CNN1
Other
null
null
null
CCOC(=O)CCNc1c2ccc(Cl)cc2nc2c(=O)[nH][nH]c(=O)c12>>O=C(O)CCNc1c2ccc(Cl)cc2nc2c(=O)[nH][nH]c(=O)c12
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-3dd4f599f9304ea3aa6b0fcf1031451d
CCOC(=O)CCN.NNc1c2ccc(Cl)cc2nc2c(=O)[nH][nH]c(=O)c12>>CCOC(=O)CCNc1c2ccc(Cl)cc2nc2c(=O)[nH][nH]c(=O)c12
Cl.ClC=1C=CC=2C(=C3C(=NC2C1)C(NNC3=O)=O)NN.Cl.C(C)OC(CCN)=O>>C(C)OC(=O)CCNC1=C2C(=NC=3C=C(C=CC13)Cl)C(NNC2=O)=O
[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][CH2:7][NH2:8].NN[c:9]1[c:10]2[cH:11][cH:12][c:13]([Cl:14])[cH:15][c:16]2[n:17][c:18]2[c:19](=[O:20])[nH:21][nH:22][c:23](=[O:24])[c:25]12>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][CH2:7][NH:8][c:9]1[c:10]2[cH:11][cH:12][c:13]([Cl:14])[cH:15][c:16]2[n:17][c:18]2[c:19](=[O:20])[nH:2...
CCOC(=O)CCN.NNc1c2ccc(Cl)cc2nc2c(=O)[nH][nH]c(=O)c12
CCOC(=O)CCNc1c2ccc(Cl)cc2nc2c(=O)[nH][nH]c(=O)c12
null
null
N1=CC=CC=C1.O
Heteroatom Alkylation and Arylation
OtherReaction
f98d784ec192c3194744583e79effe31cacfed7ba6bd47589340e7ccc1df453b
5f0b2233a04d0388eef58efc20aa7249a5468ae58d751d6d6865b0a04a6912a5
O=c1[nH][nH]c(=O)c2nc3ccccc3cc12
N-N-[c;H0;D3;+0:1]1:[c:2](:[c:3]):[c:4](:[c:5]):[#7;a:6]:[c:7]2:[c:8]:[#7;a:9]:[#7;a:10]:[c:11](=[O;D1;H0:12]):[c:13]:2:1.[#8:14]-[C:15](=[O;D1;H0:16])-[C:17]-[C:18]-[NH2;D1;+0:19]>>[#8:14]-[C:15](=[O;D1;H0:16])-[C:17]-[C:18]-[NH;D2;+0:19]-[c;H0;D3;+0:1]1:[c:2](:[c:3]):[c:4](:[c:5]):[#7;a:6]:[c:7]2:[c:8]:[#7;a:9]:[#7;a...
13
[{"value": 13.0, "product": "C(C)OC(=O)CCNC1=C2C(=NC=3C=C(C=CC13)Cl)C(NNC2=O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 11.3, "product": "C(C)OC(=O)CCNC1=C2C(=NC=3C=C(C=CC13)Cl)C(NNC2=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 7-chloro-2,3-dihydro-10-hydrazinopyridazino[4,5-b]quinoline-1,4-dione hydrochloride (1.0 g, 2.9 mM, as prepared in Example 44) and beta alanine ethyl ester hydrochloride (49.0 g, 320 mM) in pyridine (52 mL) was refluxed for 23 hr. After cooling, the vigorously stirred reaction mixture was diluted slowly wi...
10.6084/m9.figshare.5104873.v1
null
Hydrazine.Primary amine
Secondary amine
C1=c2cc3ccccc3nc2=CNN1
C1=c2cc3ccccc3nc2=CNN1
C1=c2cc3ccccc3nc2=CNN1
Other
N1=CC=CC=C1.O
null
null
CCOC(=O)CCN.NNc1c2ccc(Cl)cc2nc2c(=O)[nH][nH]c(=O)c12>N1=CC=CC=C1.O>CCOC(=O)CCNc1c2ccc(Cl)cc2nc2c(=O)[nH][nH]c(=O)c12
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-94d9309832e348ba9c46db768414dfd5
O=c1[nH][nH]c(=O)c2c(O)c3ccc(Br)cc3nc12>>O=c1[nH][nH]c(=O)c2c(O)c3ccc(Br)cc3nc12
BrC=1C=CC=2C(=C3C(=NC2C1)C(NNC3=O)=O)O.[OH-].OCC[N+](C)(C)C>>OCC[N+](C)(C)C.BrC=1C=CC=2C(=C3C(=NC2C1)C(NNC3=O)=O)O
[O:8]=[c:9]1[nH:10][nH:11][c:12](=[O:13])[c:14]2[c:15]([OH:16])[c:17]3[cH:18][cH:19][c:20]([Br:21])[cH:22][c:23]3[n:24][c:25]12>>[O:8]=[c:9]1[nH:10][nH:11][c:12](=[O:13])[c:14]2[c:15]([OH:16])[c:17]3[cH:18][cH:19][c:20]([Br:21])[cH:22][c:23]3[n:24][c:25]12
O=c1[nH][nH]c(=O)c2c(O)c3ccc(Br)cc3nc12
O=c1[nH][nH]c(=O)c2c(O)c3ccc(Br)cc3nc12
null
null
CO
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
O=c1[nH][nH]c(=O)c2nc3ccccc3cc12
null
78
[{"value": 78.0, "product": "OCC[N+](C)(C)C.BrC=1C=CC=2C(=C3C(=NC2C1)C(NNC3=O)=O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 77.2, "product": "OCC[N+](C)(C)C.BrC=1C=CC=2C(=C3C(=NC2C1)C(NNC3=O)=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a suspension of 7-bromo-2,3-dihydro-10-hydroxypyridazino[4,5-b]quinoline-1,4-dione (0.600g, 1.95 mM) in methanol (20 mL) was added choline hydroxide (0.24 g, 1.98 mM, 45% solution in methanol). The resulting solution was concentrated and the solid yellow residue was recrystallized from ethanol to provide (0.62 g, 78...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
C1=c2cc3ccccc3nc2=CNN1
null
CO
null
null
O=c1[nH][nH]c(=O)c2c(O)c3ccc(Br)cc3nc12>CO>O=c1[nH][nH]c(=O)c2c(O)c3ccc(Br)cc3nc12
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-0a45a609ac2e45e08721ea94db9274b3
CC(C)[C@H](NC(=O)OC(C)(C)C)C(N)=O.COc1ccc(P2(=S)SP(=S)(c3ccc(OC)cc3)S2)cc1>>CC(C)[C@H](NC(=O)OC(C)(C)C)C(N)=S
C(=O)(OC(C)(C)C)N[C@@H](C(C)C)C(=O)N.COC=1C=CC(=CC1)P2(=S)SP(=S)(S2)C=3C=CC(=CC3)OC>>C(=O)(OC(C)(C)C)N[C@@H](C(C)C)C(N)=S
O=[C:13]([C@H:4]([CH:2]([CH3:1])[CH3:3])[NH:5][C:6](=[O:7])[O:8][C:9]([CH3:10])([CH3:11])[CH3:12])[NH2:14].COc1ccc(P2(=S)SP(c3ccc(OC)cc3)(=[S:15])S2)cc1>>[CH3:1][CH:2]([CH3:3])[C@H:4]([NH:5][C:6](=[O:7])[O:8][C:9]([CH3:10])([CH3:11])[CH3:12])[C:13]([NH2:14])=[S:15]
CC(C)[C@H](NC(=O)OC(C)(C)C)C(N)=O.COc1ccc(P2(=S)SP(=S)(c3ccc(OC)cc3)S2)cc1
CC(C)[C@H](NC(=O)OC(C)(C)C)C(N)=S
null
null
C1CCOC1
Heteroatom Alkylation and Arylation
OtherReaction
613c2435b38505a097e2fde19577156c7ebdf46c5ee2d9d02c5db3750225691b
bad40f822f57ef1603ddc3833f08662df4bfc24add9b681d08e1ec3f67723ed7
null
C-O-c1:c:c:c(-P2(=S)-S-P(=[S;H0;D1;+0:1])(-c3:c:c:c(-O-C):c:c:3)-S-2):c:c:1.O=[C;H0;D3;+0:2](-[N;D1;H2:3])-[C:4](-[C:5])-[#7:6]-[C:7](=[O;D1;H0:8])-[#8:9]-[C:10](-[C;D1;H3:11])(-[C;D1;H3:12])-[C;D1;H3:13]>>[C:5]-[C:4](-[#7:6]-[C:7](=[O;D1;H0:8])-[#8:9]-[C:10](-[C;D1;H3:11])(-[C;D1;H3:12])-[C;D1;H3:13])-[C;H0;D3;+0:2](-...
70
[{"value": 70.0, "product": "C(=O)(OC(C)(C)C)N[C@@H](C(C)C)C(N)=S", "details": "PERCENTYIELD", "is_desired": false}, {"value": 69.4, "product": "C(=O)(OC(C)(C)C)N[C@@H](C(C)C)C(N)=S", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
Boc-valineamide (0.5 g) was stirred in dry THF at room temperature under argon. Lawesson's reagent (1.56 g, 0.6 eq) was added and the mixture was stirred overnight. The solvent was evaporated and the residue chromatographed (silica, 2.5% methanol/dichloromethane) to give the title compound as a white solid (0.373 g, 70...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Primary amide.Monosulfide.Monosulfide
Thioamide
c1ccccc1.P1SPS1.c1ccccc1
null
null
Other
C1CCOC1
null
8
CC(C)[C@H](NC(=O)OC(C)(C)C)C(N)=O.COc1ccc(P2(=S)SP(=S)(c3ccc(OC)cc3)S2)cc1>C1CCOC1>CC(C)[C@H](NC(=O)OC(C)(C)C)C(N)=S
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-b0f251ba8a8b43138ec22405d9b99942
CC(C)(C)[Si](C)(C)Cl.O[C@@H]1CCC[C@H]1O>>CC(C)(C)[Si](C)(C)O[C@@H]1CCC[C@H]1O
[C@@H]1([C@@H](CCC1)O)O.[Si](C)(C)(C(C)(C)C)Cl.N1C=NC=C1>>O([Si](C)(C)C(C)(C)C)[C@H]1[C@@H](CCC1)O
Cl[Si:5]([C:2]([CH3:1])([CH3:3])[CH3:4])([CH3:6])[CH3:7].[OH:8][C@@H:9]1[CH2:10][CH2:11][CH2:12][C@H:13]1[OH:14]>>[CH3:1][C:2]([CH3:3])([CH3:4])[Si:5]([CH3:6])([CH3:7])[O:8][C@@H:9]1[CH2:10][CH2:11][CH2:12][C@H:13]1[OH:14]
CC(C)(C)[Si](C)(C)Cl.O[C@@H]1CCC[C@H]1O
CC(C)(C)[Si](C)(C)O[C@@H]1CCC[C@H]1O
null
null
CN(C)C=O
Protection
Alcohol protection with silyl ethers
e19079a85b3e2f818dbb25a774b915f0e7349126f5b76d72c22f1c90edfa8480
16de9d9d08d1cc67ec96e76fc213a6b49c0af7979ac901a377ee705ba5071899
C1CCCC1
Cl-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[C:4](-[C;D1;H3:5])(-[C;D1;H3:6])-[C;D1;H3:7].[C:8]-[C:9](-[OH;D1;+0:10])-[C:11]>>[C:8]-[C:9](-[O;H0;D2;+0:10]-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[C:4](-[C;D1;H3:5])(-[C;D1;H3:6])-[C;D1;H3:7])-[C:11]
null
[]
25
CELSIUS
8
HOUR
To a mixture of t-butyldimethylsilyl chloride (5.08 g, 33.7 mmol) and imidazole (2.30 g, 33.7 mmol) in DMF (10 mL), a solution of trans-1,2-cyclopentanediol in DMF (4 mL) was added. The reaction mixture was stirred overnight at 25° C. The reaction mixture was diluted with ice water and extracted with ether. The ether e...
10.6084/m9.figshare.5104873.v1
null
Secondary alcohol.Silyl protective group
TMS ether protective group
null
null
C1CCCC1
HCl
CN(C)C=O
25
8
CC(C)(C)[Si](C)(C)Cl.O[C@@H]1CCC[C@H]1O>CN(C)C=O>CC(C)(C)[Si](C)(C)O[C@@H]1CCC[C@H]1O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-9364a4a06ced401991545a8820488b8f
[Li][CH2]CCC.c1ccc(COCn2ccnc2)cc1>>CC(C)C(O)c1nccn1COCc1ccccc1
C(C1=CC=CC=C1)OCN1C=NC=C1.C1CCOC1.[Li]CCCC>>C(C1=CC=CC=C1)OCN1C(=NC=C1)C(C(C)C)O
[Li][CH2][CH2:1][CH2:2][CH3:3].[cH:6]1[n:7][cH:8][cH:9][n:10]1[CH2:11][O:12][CH2:13][c:14]1[cH:15][cH:16][cH:17][cH:18][cH:19]1>>[CH3:1][CH:2]([CH3:3])[CH:4]([OH:5])[c:6]1[n:7][cH:8][cH:9][n:10]1[CH2:11][O:12][CH2:13][c:14]1[cH:15][cH:16][cH:17][cH:18][cH:19]1
[Li][CH2]CCC.c1ccc(COCn2ccnc2)cc1
CC(C)C(O)c1nccn1COCc1ccccc1
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
831678e4cbc436395546aca685c7c5e29bb63644a93b6ae8aa2e54462c0cc0e9
4ccdf76089dbbce498de631b1bc2db02ddd1c7c47d40bd0396e240884451beff
c1ccc(COCn2ccnc2)cc1
[C;D1;H3:1]-[CH2;D2;+0:2]-[CH2;D2;+0:3]-[CH2]-[Li].[C:4]-[#7;a:5]1:[c:6]:[c:7]:[#7;a:8]:[cH;D2;+0:9]:1>>[C:4]-[#7;a:5]1:[c:6]:[c:7]:[#7;a:8]:[c;H0;D3;+0:9]:1-[C:10](-[O;D1;H1:11])-[CH;D3;+0:2](-[C;D1;H3:1])-[CH3;D1;+0:3]
69
[{"value": 69.0, "product": "C(C1=CC=CC=C1)OCN1C(=NC=C1)C(C(C)C)O", "details": "PERCENTYIELD", "is_desired": false}]
-40
CELSIUS
15
MINUTE
1-benzyloxymethylimidazole prepared according to the procedure of Ngochindo, R., J. Chem. Res. (S), 58 (1990)) (3.76 g, 20 mmol), and THF (40 mL) at -40° C., was treated dropwise with n-BuLi (8.4 mL, 21 mmol, 2.5M in hexane). The resulting solution was stirred at -40° C. for 15 min, and i-butyraldehyde (2.0 mL, 22 mmol...
10.6084/m9.figshare.5104873.v1
null
Alkyl lithium
Secondary alcohol
c1c[nH]cn1
c1ncc[nH]1
c1ncc[nH]1.c1ccccc1
null
O
-40
0.25
[Li][CH2]CCC.c1ccc(COCn2ccnc2)cc1>O>CC(C)C(O)c1nccn1COCc1ccccc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-af96ced584d54df9885b41c24ce0e973
CC(=O)OC(C)(C)C.CC(C)C(=O)c1nc(COCc2ccccc2)c[nH]1>>CC(C)C(O)(CC(=O)OC(C)(C)C)c1nccn1COCc1ccccc1
CN(C)P(=O)(N(C)C)N(C)C.C(=O)([O-])[O-].[K+].[K+].C(C)(=O)OC(C)(C)C.[Li]CCCC.C(C1=CC=CC=C1)OCC=1N=C(NC1)C(C(C)C)=O.C(C)(C)NC(C)C>>C(C1=CC=CC=C1)OCN1C(=NC=C1)C(CC(=O)OC(C)(C)C)(C(C)C)O
[CH3:6][C:7](=[O:8])[O:9][C:10]([CH3:11])([CH3:12])[CH3:13].[CH3:1][CH:2]([CH3:3])[C:4](=[O:5])[c:14]1[n:15][c:16]([CH2:19][O:20][CH2:21][c:22]2[cH:23][cH:24][cH:25][cH:26][cH:27]2)[cH:17][nH:18]1>>[CH3:1][CH:2]([CH3:3])[C:4]([OH:5])([CH2:6][C:7](=[O:8])[O:9][C:10]([CH3:11])([CH3:12])[CH3:13])[c:14]1[n:15][cH:16][cH:17...
CC(=O)OC(C)(C)C.CC(C)C(=O)c1nc(COCc2ccccc2)c[nH]1
CC(C)C(O)(CC(=O)OC(C)(C)C)c1nccn1COCc1ccccc1
null
null
C1CCOC1
Heteroatom Alkylation and Arylation
OtherReaction
d9dc4e073f3bc32a587d45cd9254c140ef04fd88ac7b2286fe9f047820f70927
74b8d38f3ae0a76226c0d6ae6220b5ec0c4d96c96094da6befdb2ae8e1120e84
c1ccc(COCn2ccnc2)cc1
[C;D1;H3:1]-[C:2](-[C;D1;H3:3])(-[C;D1;H3:4])-[#8:5]-[C:6](-[CH3;D1;+0:7])=[O;D1;H0:8].[C:9]-[#8:10]-[CH2;D2;+0:11]-[c;H0;D3;+0:12]1:[#7;a:13]:[c:14](-[C;H0;D3;+0:15](=[O;H0;D1;+0:16])-[C:17](-[C;D1;H3:18])-[C;D1;H3:19]):[nH;D2;+0:20]:[c:21]:1>>[C:9]-[#8:10]-[CH2;D2;+0:11]-[n;H0;D3;+0:20]1:[c:21]:[cH;D2;+0:12]:[#7;a:13...
90
[{"value": 90.0, "product": "C(C1=CC=CC=C1)OCN1C(=NC=C1)C(CC(=O)OC(C)(C)C)(C(C)C)O", "details": "PERCENTYIELD", "is_desired": false}]
-10
CELSIUS
null
null
Diisopropylamine (83 μL, 0.59 mmol) and THF (1.5 mL) were cooled to -40° C. and n-BuLi (188 μL, 0.47 mmol, 2.5M in hexane) was added. The reaction mixture was warmed to -10° C. and stirred for 15 m, recooled to -70° C. and t-butyl acetate (63 μL, 0.47 mmol) was added. The reaction was stirred for 5 m, and HMPA (254 μL,...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ester.Ether
Ester.Ether.Tertiary alcohol
c1c[nH]cn1
c1ncc[nH]1
c1ncc[nH]1.c1ccccc1
null
C1CCOC1
-10
null
CC(=O)OC(C)(C)C.CC(C)C(=O)c1nc(COCc2ccccc2)c[nH]1>C1CCOC1>CC(C)C(O)(CC(=O)OC(C)(C)C)c1nccn1COCc1ccccc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-0fb4566f15574ed1bc3456297724c43f
CCOC(=O)c1cc2ccccc2n(C(C)C)c1=O>>CC(C)n1c(=O)c(C(=O)O)cc2ccccc21
C(C)(C)N1C(C(=CC2=CC=CC=C12)C(=O)OCC)=O.[OH-].[Na+].C(C)O>>C(C)(C)N1C(C(=CC2=CC=CC=C12)C(=O)O)=O
CC[O:10][C:8]([c:7]1[c:5](=[O:6])[n:4]([CH:2]([CH3:1])[CH3:3])[c:17]2[c:12]([cH:11]1)[cH:13][cH:14][cH:15][cH:16]2)=[O:9]>>[CH3:1][CH:2]([CH3:3])[n:4]1[c:5](=[O:6])[c:7]([C:8](=[O:9])[OH:10])[cH:11][c:12]2[cH:13][cH:14][cH:15][cH:16][c:17]12
CCOC(=O)c1cc2ccccc2n(C(C)C)c1=O
CC(C)n1c(=O)c(C(=O)O)cc2ccccc21
null
null
O
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=c1ccc2ccccc2[nH]1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]:[#7;a:6]>>[#7;a:6]:[c:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
88.3
[{"value": 88.3, "product": "C(C)(C)N1C(C(=CC2=CC=CC=C12)C(=O)O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
A solution of 1.55 g of ethyl 1-isopropyl-2(1H)-quinolone-3-carboxylate and 0.28 g of sodium hydroxide in a solvent mixture of 10 ml of ethanol and 2 ml of water was stirred at room temperature overnight. The solvent was evaporated under reduced pressure, and after addition of dil. hydrochloric acid, the precipitated s...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccc2ncccc2c1
Other
O
null
8
CCOC(=O)c1cc2ccccc2n(C(C)C)c1=O>O>CC(C)n1c(=O)c(C(=O)O)cc2ccccc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-8547a040ad9a425c98f22d4b4c6c403c
CC(C)Nc1ccccc1CO>>CC(C)Nc1ccccc1C=O
C(C)(C)NC1=C(CO)C=CC=C1.ClC=1C(C(=C(C(C1Cl)=O)C#N)C#N)=O>>C(C)(C)NC1=C(C=O)C=CC=C1
[CH3:1][CH:2]([CH3:3])[NH:4][c:5]1[cH:6][cH:7][cH:8][cH:9][c:10]1[CH2:11][OH:12]>>[CH3:1][CH:2]([CH3:3])[NH:4][c:5]1[cH:6][cH:7][cH:8][cH:9][c:10]1[CH:11]=[O:12]
CC(C)Nc1ccccc1CO
CC(C)Nc1ccccc1C=O
null
null
O1CCOCC1
Oxidation
Oxidation or Dehydrogenation of Alcohols to Aldehydes and Ketones
41bfa9deea81b465c88ad21fdfb64a2e1ba29490558cf430df132cb98b4a538b
0a03c6724c1862e8f86d4a463afda55b8e067dc6cb42597b472eb7cabc03eda3
c1ccccc1
[OH;D1;+0:1]-[CH2;D2;+0:2]-[c:3](:[c:4]):[c:5]>>[O;H0;D1;+0:1]=[CH;D2;+0:2]-[c:3](:[c:4]):[c:5]
80.1
[{"value": 80.1, "product": "C(C)(C)NC1=C(C=O)C=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of 9.6 g of 2-isopropylaminobenzyl alcohol in 200 ml of dioxane was added 13.2 g of 2,3-dichloro-5,6-dicyano-1,4-benzoquinone (DDQ) in several portions, followed by stirring for an hour. The solvent was evaporated, the reaction solution was concentrated, and methylene chloride was added thereto, followed ...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Aldehyde
null
null
c1ccccc1
null
O1CCOCC1
null
null
CC(C)Nc1ccccc1CO>O1CCOCC1>CC(C)Nc1ccccc1C=O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-6ea71cac5fe24314936a22d13c05f389
CC(C)Nc1ccccc1C=O.CCOC(=O)CC(=O)OCC>>CCOC(=O)c1cc2ccccc2n(C(C)C)c1=O
C(C)(C)NC1=C(C=O)C=CC=C1.C(CC(=O)OCC)(=O)OCC.C([O-])(O)=O.[Na+]>>C(C)(C)N1C(C(=CC2=CC=CC=C12)C(=O)OCC)=O
O=[CH:7][c:8]1[cH:9][cH:10][cH:11][cH:12][c:13]1[NH:14][CH:15]([CH3:16])[CH3:17].CCO[C:18]([CH2:6][C:4]([O:3][CH2:2][CH3:1])=[O:5])=[O:19]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]2[n:14]([CH:15]([CH3:16])[CH3:17])[c:18]1=[O:19]
CC(C)Nc1ccccc1C=O.CCOC(=O)CC(=O)OCC
CCOC(=O)c1cc2ccccc2n(C(C)C)c1=O
null
null
C(C)(=O)OC(C)=O
Aromatic Heterocycle Formation
OtherReaction
729ffe8850d05b6f2f8f8601c180def2bd405d714b65f772032554626ca5b59d
e01ead31c330dcfd1f5449feed0e578553ffcacb3b875032b5383c9a1ab25b8b
O=c1ccc2ccccc2[nH]1
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[CH2;D2;+0:3]-[C:4](=[O;D1;H0:5])-[#8:6]-[C:7].O=[CH;D2;+0:8]-[c:9](:[c:10]):[c:11](-[NH;D2;+0:12]-[C:13](-[C;D1;H3:14])-[C;D1;H3:15]):[c:16]>>[C:7]-[#8:6]-[C:4](=[O;D1;H0:5])-[c;H0;D3;+0:3]1:[cH;D2;+0:8]:[c:9](:[c:10]):[c:11](:[c:16]):[n;H0;D3;+0:12](-[C:13](-[C;D1;H3:14])-[C;D1;H3:1...
61.3
[{"value": 61.3, "product": "C(C)(C)N1C(C(=CC2=CC=CC=C12)C(=O)OCC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
null
null
A solution of 7.5 g of 2-isopropylaminobenzaldehyde, 11.0 g of diethyl malonate and 11.6 g of sodium bicarbonate in 800 ml of acetic anhydride was stirred under heating at 100° C. for 15 hours. After evaporation of the solvent under reduced pressure, water was added, followed by extraction with ethyl acetate. The organ...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Ester.Ester.Secondary amine
Ester
c1ccccc1
c1ccc2ncccc2c1
c1ccc2ncccc2c1
HO-
C(C)(=O)OC(C)=O
100
null
CC(C)Nc1ccccc1C=O.CCOC(=O)CC(=O)OCC>C(C)(=O)OC(C)=O>CCOC(=O)c1cc2ccccc2n(C(C)C)c1=O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-18f7f5d0bdf24923973a1222b73ecdad
CCOC(=O)c1c(-c2ccc3c(c2)OCO3)c2ccccc2[nH]c1=O>>O=C(O)c1c(-c2ccc3c(c2)OCO3)c2ccccc2[nH]c1=O
Cl.C(C)OC(=O)C=1C(NC2=CC=CC=C2C1C1=CC2=C(C=C1)OCO2)=O.CO.[OH-].[K+]>>C1OC=2C=C(C=CC2O1)C1=C(C(NC2=CC=CC=C12)=O)C(=O)O
CC[O:3][C:2](=[O:1])[c:4]1[c:5](-[c:6]2[cH:7][cH:8][c:9]3[c:10]([cH:11]2)[O:12][CH2:13][O:14]3)[c:15]2[cH:16][cH:17][cH:18][cH:19][c:20]2[nH:21][c:22]1=[O:23]>>[O:1]=[C:2]([OH:3])[c:4]1[c:5](-[c:6]2[cH:7][cH:8][c:9]3[c:10]([cH:11]2)[O:12][CH2:13][O:14]3)[c:15]2[cH:16][cH:17][cH:18][cH:19][c:20]2[nH:21][c:22]1=[O:23]
CCOC(=O)c1c(-c2ccc3c(c2)OCO3)c2ccccc2[nH]c1=O
O=C(O)c1c(-c2ccc3c(c2)OCO3)c2ccccc2[nH]c1=O
null
null
O
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=c1cc(-c2ccc3c(c2)OCO3)c2ccccc2[nH]1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]:[#7;a:6]>>[#7;a:6]:[c:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
95.4
[{"value": 95.4, "product": "C1OC=2C=C(C=CC2O1)C1=C(C(NC2=CC=CC=C12)=O)C(=O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 95.4, "product": "C1OC=2C=C(C=CC2O1)C1=C(C(NC2=CC=CC=C12)=O)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 1,2-dihydro-4-(3,4-methylenedioxyphenyl)-2-oxo-3-quinoline carboxylic acid ethyl ester (40 g, 118.6 mmol), methanol (200 ml), water (300 ml) and potassium hydroxide (33.3 g, 593.5 mmol) was refluxed with heat for 40 hours. To the reaction mixture was added 110 ml of 6N-HCl to acidify the mixture to obtain ...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccc2c(c1)OCO2.c1cnc2ccccc2c1
Other
O
null
null
CCOC(=O)c1c(-c2ccc3c(c2)OCO3)c2ccccc2[nH]c1=O>O>O=C(O)c1c(-c2ccc3c(c2)OCO3)c2ccccc2[nH]c1=O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-08a65d3d86274d87908614df5eeda1f8
O=C(O)c1c(-c2ccc3c(c2)OCO3)c2ccccc2[nH]c1=O.O=P(Cl)(Cl)Cl>>O=C1c2cc3c(cc2-c2c1c(Cl)nc1ccccc21)OCO3
C1OC=2C=C(C=CC2O1)C1=C(C(NC2=CC=CC=C12)=O)C(=O)O.P(=O)(Cl)(Cl)Cl>>ClC1=NC2=CC=CC=C2C2=C1C(C1=CC3=C(C=C12)OCO3)=O
O=[c:11]1[c:10]([C:2](O)=[O:1])[c:9](-[c:8]2[cH:3][cH:4][c:5]3[c:6]([cH:7]2)[O:20][CH2:21][O:22]3)[c:19]2[c:14]([nH:13]1)[cH:15][cH:16][cH:17][cH:18]2.O=P(Cl)(Cl)[Cl:12]>>[O:1]=[C:2]1[c:3]2[cH:4][c:5]3[c:6]([cH:7][c:8]2-[c:9]2[c:10]1[c:11]([Cl:12])[n:13][c:14]1[cH:15][cH:16][cH:17][cH:18][c:19]21)[O:20][CH2:21][O:22]3
O=C(O)c1c(-c2ccc3c(c2)OCO3)c2ccccc2[nH]c1=O.O=P(Cl)(Cl)Cl
O=C1c2cc3c(cc2-c2c1c(Cl)nc1ccccc21)OCO3
null
null
O1CCCC1
Functional Group Interconversion
OtherReaction
543e37a7a1f36d75ee988a367790d70acab5cef0bd77b8e407415edb03f42eb1
3222cccc60f66cbdb8ac8bb7a1f67e9f671c77d8cc441c4fc8b05ddd04bfbcfc
O=C1c2cc3c(cc2-c2c1cnc1ccccc21)OCO3
Cl-P(-Cl)(=O)-[Cl;H0;D1;+0:1].O-[C;H0;D3;+0:2](=[O;D1;H0:3])-[c:4]1:[c:5](-[c:6](:[c:7]):[cH;D2;+0:8]:[c:9]:[c:10]-[#8:11]):[c:12]:[c:13](:[c:14]):[nH;D2;+0:15]:[c;H0;D3;+0:16]:1=O>>[#8:11]-[c:10]:[c:9]:[c;H0;D3;+0:8]1:[c:6](:[c:7])-[c:5]2:[c:12]:[c:13](:[c:14]):[n;H0;D2;+0:15]:[c;H0;D3;+0:16](-[Cl;H0;D1;+0:1]):[c:4]:2...
59.9
[{"value": 59.9, "product": "ClC1=NC2=CC=CC=C2C2=C1C(C1=CC3=C(C=C12)OCO3)=O", "details": "PERCENTYIELD", "is_desired": false}]
90
CELSIUS
null
null
A mixture of 1,2-dihydro-4-(3,4-methylenedioxyphenyl)-2-oxo-3-quinoline carboxylic acid obtained in reference example 1 (10 g, 32.3 mmol) and phosphorous oxychloride (100 ml, 1.07 mol) was refluxed with heat for 4 hours. The reaction mixture was distilled to dryness and washed with n-hexane several times. To the residu...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Aromatic halide.Ketone
c1ccc2c(c1)OCO2.c1cnc2ccccc2c1
c1ccc2c(c1)ncc1c2c2cc3c(cc2C1)OCO3
c1ccc2c(c1)ncc1c2c2cc3c(cc2C1)OCO3
HCl
O1CCCC1
90
null
O=C(O)c1c(-c2ccc3c(c2)OCO3)c2ccccc2[nH]c1=O.O=P(Cl)(Cl)Cl>O1CCCC1>O=C1c2cc3c(cc2-c2c1c(Cl)nc1ccccc21)OCO3
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-5080020aec3640ada6d73af7d0efbd44
CCOC(=O)c1c(-c2ccccc2)c2ccccc2[nH]c1=O>>O=C(O)c1c(-c2ccccc2)c2ccccc2[nH]c1=O
Cl.C(C)OC(=O)C=1C(NC2=CC=CC=C2C1C1=CC=CC=C1)=O.C(C)O.[OH-].[K+]>>C1(=CC=CC=C1)C1=C(C(NC2=CC=CC=C12)=O)C(=O)O
CC[O:3][C:2](=[O:1])[c:4]1[c:5](-[c:6]2[cH:7][cH:8][cH:9][cH:10][cH:11]2)[c:12]2[cH:13][cH:14][cH:15][cH:16][c:17]2[nH:18][c:19]1=[O:20]>>[O:1]=[C:2]([OH:3])[c:4]1[c:5](-[c:6]2[cH:7][cH:8][cH:9][cH:10][cH:11]2)[c:12]2[cH:13][cH:14][cH:15][cH:16][c:17]2[nH:18][c:19]1=[O:20]
CCOC(=O)c1c(-c2ccccc2)c2ccccc2[nH]c1=O
O=C(O)c1c(-c2ccccc2)c2ccccc2[nH]c1=O
null
null
O
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=c1cc(-c2ccccc2)c2ccccc2[nH]1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]:[#7;a:6]>>[#7;a:6]:[c:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
93.1
[{"value": 92.9, "product": "C1(=CC=CC=C1)C1=C(C(NC2=CC=CC=C12)=O)C(=O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 93.1, "product": "C1(=CC=CC=C1)C1=C(C(NC2=CC=CC=C12)=O)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 1,2-dihydro-4-phenyl-2-oxo-3-quinoline carboxylic acid ethyl ester (5 g, 17 mmol), ethanol (20 ml), water (40 ml) and potassium hydroxide (5 g, mmol) was refluxed with heat for 1.5 hours. To the reaction mixture was added 60 ml of 2N-HCl to acidify the mixture to obtain a precipitated crystal by filtration...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1cnc2ccccc2c1
Other
O
null
null
CCOC(=O)c1c(-c2ccccc2)c2ccccc2[nH]c1=O>O>O=C(O)c1c(-c2ccccc2)c2ccccc2[nH]c1=O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-40686f94c8ff48678189869d94122470
CCOC(=O)c1c(-c2ccccc2)c2ccc(C)cc2[nH]c1=O>>Cc1ccc2c3c(c(=O)[nH]c2c1)C(=O)c1ccccc1-3
C(C)OC(=O)C=1C(NC2=CC(=CC=C2C1C1=CC=CC=C1)C)=O>>CC1=CC=C2C3=C(C(NC2=C1)=O)C(C1=CC=CC=C13)=O
CCO[C:13]([c:7]1[c:6](-[c:20]2[cH:15][cH:19][cH:18][cH:17][cH:16]2)[c:5]2[cH:4][cH:3][c:2]([CH3:1])[cH:12][c:11]2[nH:10][c:8]1=[O:9])=[O:14]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]2[c:6]3[c:7]([c:8](=[O:9])[nH:10][c:11]2[cH:12]1)[C:13](=[O:14])[c:15]1[cH:16][cH:17][cH:18][cH:19][c:20]1-3
CCOC(=O)c1c(-c2ccccc2)c2ccc(C)cc2[nH]c1=O
Cc1ccc2c3c(c(=O)[nH]c2c1)C(=O)c1ccccc1-3
null
null
S(O)(O)(=O)=O
C-C Coupling
OtherReaction
74cf47bc32c60b614b02500a53806bb8f623818590d3a4063f8137ba05983240
f80cbbd7f2bfc042e62829b7de30498cf0880b808f2adad888ffdfe089982722
O=C1c2ccccc2-c2c1c(=O)[nH]c1ccccc21
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4](-[c;H0;D3;+0:5]2:[cH;D2;+0:6]:[cH;D2;+0:7]:[c:8]:[c:9]:[cH;D2;+0:10]:2):[c:11]:[c:12]:[#7;a:13]:[c:14]:1=[O;D1;H0:15]>>[O;D1;H0:2]=[C;H0;D3;+0:1]1-[c:3]2:[c:4](:[c:11]:[c:12]:[#7;a:13]:[c:14]:2=[O;D1;H0:15])-[c;H0;D3;+0:5]2:[cH;D2;+0:7]:[c:8]:[c:9]:[cH;D2;+0:10]:[c;H0;D3;...
null
[]
95
CELSIUS
null
null
A mixture of 1,2-dihydro-4-phenyl-7-methyl-2-oxo-3-quinoline carboxylic acid ethyl ester (2.5 g, 8.1 mmol) and conc. sulfuric acid (20 ml) was stirred with heat at 95° C. for 10 hours. The reaction mixture was poured into ice water to obtain a crystal precipitated by filtration. The crystal obtained was washed with wat...
10.6084/m9.figshare.5104873.v1
null
Ester
Ketone
c1ccccc1
C1c2ccccc2c2c1cnc1ccccc12
C1c2ccccc2c2c1cnc1ccccc12
HO-
S(O)(O)(=O)=O
95
null
CCOC(=O)c1c(-c2ccccc2)c2ccc(C)cc2[nH]c1=O>S(O)(O)(=O)=O>Cc1ccc2c3c(c(=O)[nH]c2c1)C(=O)c1ccccc1-3
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-d9236b54d4954b7aa9b9f3b9d4ae71c7
Cc1ccc2c3c(c(=O)[nH]c2c1)C(=O)c1ccccc1-3.O=P(Cl)(Cl)Cl>>Cc1ccc2c3c(c(Cl)nc2c1)C(=O)c1ccccc1-3
CC1=CC=C2C3=C(C(NC2=C1)=O)C(C1=CC=CC=C13)=O.P(=O)(Cl)(Cl)Cl>>ClC1=NC2=CC(=CC=C2C2=C1C(C1=CC=CC=C12)=O)C
O=[c:8]1[c:7]2[c:6]([c:5]3[cH:4][cH:3][c:2]([CH3:1])[cH:12][c:11]3[nH:10]1)-[c:20]1[c:15]([cH:16][cH:17][cH:18][cH:19]1)[C:13]2=[O:14].O=P(Cl)(Cl)[Cl:9]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]2[c:6]3[c:7]([c:8]([Cl:9])[n:10][c:11]2[cH:12]1)[C:13](=[O:14])[c:15]1[cH:16][cH:17][cH:18][cH:19][c:20]1-3
Cc1ccc2c3c(c(=O)[nH]c2c1)C(=O)c1ccccc1-3.O=P(Cl)(Cl)Cl
Cc1ccc2c3c(c(Cl)nc2c1)C(=O)c1ccccc1-3
null
null
null
Functional Group Interconversion
OtherReaction
5e9dd541e33e00251f4cb33b88e87b9d504018c590d84ac6a9372bbc42fd7bc5
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
O=C1c2ccccc2-c2c1cnc1ccccc21
Cl-P(-Cl)(=O)-[Cl;H0;D1;+0:1].O=[c;H0;D3;+0:2]1:[nH;D2;+0:3]:[c:4](:[c:5]):[c:6]:[c:7]:[c:8]:1-[C:9](=[O;D1;H0:10])-[c:11]>>[Cl;H0;D1;+0:1]-[c;H0;D3;+0:2]1:[n;H0;D2;+0:3]:[c:4](:[c:5]):[c:6]:[c:7]:[c:8]:1-[C:9](=[O;D1;H0:10])-[c:11]
73.4
[{"value": 73.4, "product": "ClC1=NC2=CC(=CC=C2C2=C1C(C1=CC=CC=C12)=O)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 3-methyl-5H-indeno[2,1-c]quinoline-6,7-dion obtained in reference example 5 (700 mg, 2.7 mmol) and phosphorous oxychloride (10 ml, 107 mmol) was refluxed with heat for 1.5 hours. The reaction mixture was distilled to dryness. To the residue was added water to obtain a crystal precipitated by filtration. Th...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
C1c2ccccc2c2c1cnc1ccccc12
c1ccc2c(c1)Cc1cnc3ccccc3c12
c1ccc2c(c1)Cc1cnc3ccccc3c12
HCl
null
null
null
Cc1ccc2c3c(c(=O)[nH]c2c1)C(=O)c1ccccc1-3.O=P(Cl)(Cl)Cl>>Cc1ccc2c3c(c(Cl)nc2c1)C(=O)c1ccccc1-3
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-c39dc7ddfdaf41718ff28171b32b7253
CCC(CC)(C(=O)[O-])C(=O)[O-].CCO.COc1ccc(C(=O)c2ccccc2)c(N)c1>>CCOC(=O)c1c(-c2ccccc2)c2ccc(OC)cc2[nH]c1=O
C(C)O.NC1=C(C(=O)C2=CC=CC=C2)C=CC(=C1)OC.C(C)C(C(=O)[O-])(C(=O)[O-])CC>>C(C)OC(=O)C=1C(NC2=CC(=CC=C2C1C1=CC=CC=C1)OC)=O
CC[C:6](CC)([C:4]([O-])=[O:5])[C:23]([O-])=[O:24].[CH3:1][CH2:2][OH:3].O=[C:7]([c:8]1[cH:9][cH:10][cH:11][cH:12][cH:13]1)[c:14]1[cH:15][cH:16][c:17]([O:18][CH3:19])[cH:20][c:21]1[NH2:22]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[c:7](-[c:8]2[cH:9][cH:10][cH:11][cH:12][cH:13]2)[c:14]2[cH:15][cH:16][c:17]([O:18][CH3:19])[c...
CCC(CC)(C(=O)[O-])C(=O)[O-].CCO.COc1ccc(C(=O)c2ccccc2)c(N)c1
CCOC(=O)c1c(-c2ccccc2)c2ccc(OC)cc2[nH]c1=O
null
null
null
Aromatic Heterocycle Formation
OtherReaction
a22b280606df717de5da2cb298275accbc9bf15ee6ef21165528469877751748
459e7381b48255c35b0f54131b1cc18a13864ee1e81675dcd1a560b0b90e67dd
O=c1cc(-c2ccccc2)c2ccccc2[nH]1
C-C-[C;H0;D4;+0:1](-C-C)(-[C;H0;D3;+0:2](-[O-])=[O;D1;H0:3])-[C;H0;D3;+0:4](-[O-])=[O;D1;H0:5].O=[C;H0;D3;+0:6](-[c:7](:[c:8]):[c:9](-[NH2;D1;+0:10]):[c:11])-[c;H0;D3;+0:12](:[c:13]:[c:14]):[c:15]:[c:16].[C;D1;H3:17]-[C:18]-[OH;D1;+0:19]>>[C;D1;H3:17]-[C:18]-[O;H0;D2;+0:19]-[C;H0;D3;+0:4](=[O;D1;H0:5])-[c;H0;D3;+0:1]1:...
90.2
[{"value": 90.2, "product": "C(C)OC(=O)C=1C(NC2=CC(=CC=C2C1C1=CC=CC=C1)OC)=O", "details": "PERCENTYIELD", "is_desired": false}]
160
CELSIUS
null
null
A mixture of 2-amino-4-methoxybenzophenone (20 g, 88 mmol), diethylmalonate (26.7 ml, 176 mmol), 1,8-diazabicyclo[5,2,0]-undeca-7-en (DBU) (0.66 ml, 4.4 mmol) was stirred with heat at 160° C. for 2 hours. The reaction mixture was cooled by air. To the cooled mixture was added ethanol (30 ml) to obtain a precipitated cr...
10.6084/m9.figshare.5104873.v1
null
Ketone.Primary alcohol.Primary amine
Ester
c1ccccc1
c1cnc2ccccc2c1
c1ccccc1.c1cnc2ccccc2c1
HO-
null
160
null
CCC(CC)(C(=O)[O-])C(=O)[O-].CCO.COc1ccc(C(=O)c2ccccc2)c(N)c1>>CCOC(=O)c1c(-c2ccccc2)c2ccc(OC)cc2[nH]c1=O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-bd6b84b0847d406aae39ab734c84c1c7
O=C1c2ccccc2-c2c1[nH]c(=O)c1ccccc21.O=P(Cl)(Cl)Cl>>O=C1c2ccccc2-c2c1nc(Cl)c1ccccc21
C1=C2C3=C(NC(C2=CC=C1)=O)C(C1=CC=CC=C13)=O.P(=O)(Cl)(Cl)Cl>>ClC1=NC2=C(C3=CC=CC=C13)C1=CC=CC=C1C2=O
O=[c:12]1[nH:11][c:10]2[c:9]([c:19]3[c:14]1[cH:15][cH:16][cH:17][cH:18]3)-[c:8]1[c:3]([cH:4][cH:5][cH:6][cH:7]1)[C:2]2=[O:1].O=P(Cl)(Cl)[Cl:13]>>[O:1]=[C:2]1[c:3]2[cH:4][cH:5][cH:6][cH:7][c:8]2-[c:9]2[c:10]1[n:11][c:12]([Cl:13])[c:14]1[cH:15][cH:16][cH:17][cH:18][c:19]21
O=C1c2ccccc2-c2c1[nH]c(=O)c1ccccc21.O=P(Cl)(Cl)Cl
O=C1c2ccccc2-c2c1nc(Cl)c1ccccc21
null
null
CN(C=O)C
Functional Group Interconversion
OtherReaction
1c742d69c8b6c3cd5770be5e58f0553876f7d2550b6be59e9046e3287dd7aaba
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
O=C1c2ccccc2-c2c1ncc1ccccc21
Cl-P(-Cl)(=O)-[Cl;H0;D1;+0:1].O=[c;H0;D3;+0:2]1:[nH;D2;+0:3]:[c:4](:[c:5]:[c:6]:[c:7]:1:[c:8])-[C:9](=[O;D1;H0:10])-[c:11]>>[Cl;H0;D1;+0:1]-[c;H0;D3;+0:2]1:[n;H0;D2;+0:3]:[c:4](:[c:5]:[c:6]:[c:7]:1:[c:8])-[C:9](=[O;D1;H0:10])-[c:11]
78.7
[{"value": 78.7, "product": "ClC1=NC2=C(C3=CC=CC=C13)C1=CC=CC=C1C2=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 6H-indeno[2,1-c]isoquinoline-5,7-dion obtained in reference example 16 (26.6 g, 108 mmol) and phosphorous oxychloride (300 ml) was refluxed with heat in the presence of 1 ml of N,N-dimethylformamide for 2 hours. The reaction mixture was distilled to dryness. To the residue was added ice water to obtain a c...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
C1c2ccccc2c2c1ncc1ccccc12
c1ccc2c(c1)Cc1ncc3ccccc3c12
c1ccc2c(c1)Cc1ncc3ccccc3c12
HCl
CN(C=O)C
null
null
O=C1c2ccccc2-c2c1[nH]c(=O)c1ccccc21.O=P(Cl)(Cl)Cl>CN(C=O)C>O=C1c2ccccc2-c2c1nc(Cl)c1ccccc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-afb2bac37106446f80150be5390395af
CN(C)CCN.O=C1c2ccccc2-c2c1c(Cl)nc1cc(F)ccc21>>CN(C)CCNc1nc2cc(F)ccc2c2c1C(=O)c1ccccc1-2.Cl.Cl
ClC1=NC2=CC(=CC=C2C2=C1C(C1=CC=CC=C12)=O)F.CN(CCN)C>>Cl.Cl.CN(C)CCNC1=NC2=CC(=CC=C2C2=C1C(C1=CC=CC=C12)=O)F
[CH3:1][N:2]([CH3:3])[CH2:4][CH2:5][NH2:6].[c:7]1([Cl:26])[n:8][c:9]2[cH:10][c:11]([F:12])[cH:13][cH:14][c:15]2[c:16]2[c:17]1[C:18](=[O:19])[c:20]1[cH:21][cH:22][cH:23][cH:24][c:25]1-2>>[CH3:1][N:2]([CH3:3])[CH2:4][CH2:5][NH:6][c:7]1[n:8][c:9]2[cH:10][c:11]([F:12])[cH:13][cH:14][c:15]2[c:16]2[c:17]1[C:18](=[O:19])[c:20...
CN(C)CCN.O=C1c2ccccc2-c2c1c(Cl)nc1cc(F)ccc21
CN(C)CCNc1nc2cc(F)ccc2c2c1C(=O)c1ccccc1-2.Cl.Cl
null
null
null
Functional Group Addition
N-arylation (Buchwald-Hartwig/Ullmann-Goldberg)
18f2f261f905c62bee5916bb9821e685b82d92037febfdc52d35c3760f226e9a
6f78585f8136bfeb64030c4a3c4021c4cf8a554288637e24070b99b83b5f9b48
O=C1c2ccccc2-c2c1cnc1ccccc21
[C:1]-[C:2]-[NH2;D1;+0:3].[Cl;H0;D1;+0:4]-[c;H0;D3;+0:5](:[#7;a:6]:[c:7]):[c:8](:[c:9])-[C:10](=[O;D1;H0:11])-[c:12]>>[C:1]-[C:2]-[NH;D2;+0:3]-[c;H0;D3;+0:5](:[#7;a:6]:[c:7]):[c:8](:[c:9])-[C:10](=[O;D1;H0:11])-[c:12].[ClH;D0;+0:4]
68.6
[{"value": 34.3, "product": "Cl.Cl.CN(C)CCNC1=NC2=CC(=CC=C2C2=C1C(C1=CC=CC=C12)=O)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 68.6, "product": "Cl.Cl.CN(C)CCNC1=NC2=CC(=CC=C2C2=C1C(C1=CC=CC=C12)=O)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
90
CELSIUS
null
null
To a suspension of 6-chloro-3-fluoro-7H-indeno[2,1-c]quinoline-7-on (860 mg, 3.0 mmol) in pyrydine (10 ml) was added N,N-dimethylethylenediamine (800 mg, 9.0 mmol), and the mixture was stirred with heat at 90° C. for 12 hours. The reaction mixture was distilled to dryness. To the residue was added water and chloroform ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1ccc2c(c1)Cc1cnc3ccccc3c12
c1ccc2c(c1)Cc1cnc3ccccc3c12
c1ccc2c(c1)Cc1cnc3ccccc3c12
Other
null
90
null
CN(C)CCN.O=C1c2ccccc2-c2c1c(Cl)nc1cc(F)ccc21>>CN(C)CCNc1nc2cc(F)ccc2c2c1C(=O)c1ccccc1-2.Cl.Cl
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-7a2a319b1424424183bfefb01280793f
COc1ccc2c3c(c(NCCN(C)C)nc2c1)C(=O)c1ccccc1-3>>CN(C)CCNc1nc2cc(O)ccc2c2c1C(=O)c1ccccc1-2
CN(C)CCNC1=NC2=CC(=CC=C2C2=C1C(C1=CC=CC=C12)=O)OC.Br>>CN(C)CCNC1=NC2=CC(=CC=C2C2=C1C(C1=CC=CC=C12)=O)O
C[O:12][c:11]1[cH:10][c:9]2[n:8][c:7]([NH:6][CH2:5][CH2:4][N:2]([CH3:1])[CH3:3])[c:17]3[c:16]([c:15]2[cH:14][cH:13]1)-[c:25]1[c:20]([cH:21][cH:22][cH:23][cH:24]1)[C:18]3=[O:19]>>[CH3:1][N:2]([CH3:3])[CH2:4][CH2:5][NH:6][c:7]1[n:8][c:9]2[cH:10][c:11]([OH:12])[cH:13][cH:14][c:15]2[c:16]2[c:17]1[C:18](=[O:19])[c:20]1[cH:2...
COc1ccc2c3c(c(NCCN(C)C)nc2c1)C(=O)c1ccccc1-3
CN(C)CCNc1nc2cc(O)ccc2c2c1C(=O)c1ccccc1-2
null
null
C(C)(=O)O
Deprotection
Cleavage of methoxy ethers to alcohols
c5320c7dfa4f544d4900efcae9b3262bf0d5286bcf39c86109232351f35b23d5
26a36596df80ec137b0e8087297418351c93c32819177f680675220622f215d4
O=C1c2ccccc2-c2c1cnc1ccccc21
C-[O;H0;D2;+0:1]-[c:2](:[c:3]):[c:4]:[c:5]:[#7;a:6]>>[#7;a:6]:[c:5]:[c:4]:[c:2](-[OH;D1;+0:1]):[c:3]
73.2
[{"value": 73.0, "product": "CN(C)CCNC1=NC2=CC(=CC=C2C2=C1C(C1=CC=CC=C12)=O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 73.2, "product": "CN(C)CCNC1=NC2=CC(=CC=C2C2=C1C(C1=CC=CC=C12)=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of 6-(((dimethylamino)ethyl)amino)-3-methoxy-7H-indeno[2,1-c]quinoline-7-on obtained in example 1 (3 g, 8.6 mmol) in acetic acid (40 ml) was added 47% aqueous hydrobromic acid (40 ml), and the mixture was refluxed with heat for 60 hours. The reaction mixture was distilled to dryness. To the residue was ad...
10.6084/m9.figshare.5104873.v1
null
Ether
Aromatic alcohol
null
null
c1ccc2c(c1)Cc1cnc3ccccc3c12
Other
C(C)(=O)O
null
null
COc1ccc2c3c(c(NCCN(C)C)nc2c1)C(=O)c1ccccc1-3>C(C)(=O)O>CN(C)CCNc1nc2cc(O)ccc2c2c1C(=O)c1ccccc1-2
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-c99b877e128f477eb3b3215ab9fd97e9
CC(C)(C)C(=O)Cl.CN(C)CCNc1nc2cc(O)ccc2c2c1C(=O)c1ccccc1-2>>CN(C)CCNc1nc2cc(OC(=O)C(C)(C)C)ccc2c2c1C(=O)c1ccccc1-2
CN(C)CCNC1=NC2=CC(=CC=C2C2=C1C(C1=CC=CC=C12)=O)O.C(C(C)(C)C)(=O)Cl.O>>CN(C)CCNC1=NC2=CC(=CC=C2C2=C1C(C1=CC=CC=C12)=O)OC(C(C)(C)C)=O
Cl[C:13](=[O:14])[C:15]([CH3:16])([CH3:17])[CH3:18].[CH3:1][N:2]([CH3:3])[CH2:4][CH2:5][NH:6][c:7]1[n:8][c:9]2[cH:10][c:11]([OH:12])[cH:19][cH:20][c:21]2[c:22]2[c:23]1[C:24](=[O:25])[c:26]1[cH:27][cH:28][cH:29][cH:30][c:31]1-2>>[CH3:1][N:2]([CH3:3])[CH2:4][CH2:5][NH:6][c:7]1[n:8][c:9]2[cH:10][c:11]([O:12][C:13](=[O:14]...
CC(C)(C)C(=O)Cl.CN(C)CCNc1nc2cc(O)ccc2c2c1C(=O)c1ccccc1-2
CN(C)CCNc1nc2cc(OC(=O)C(C)(C)C)ccc2c2c1C(=O)c1ccccc1-2
null
CN(C1=CC=NC=C1)C
ClCCl
Acylation
Schotten-Baumann to ester
1cda078f55e64d9385e544d1067595d5e7672bbd1eff542e7a341817a2d8c4d5
6439fc27f97ee9ed7c11ef9b5032d9493d05f28a7bbb50d256a2d54d035fbfb2
O=C1c2ccccc2-c2c1cnc1ccccc21
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])(-[C;D1;H3:5])-[C;D1;H3:6].[#7;a:7]:[c:8]:[c:9]:[c:10](-[OH;D1;+0:11]):[c:12]>>[#7;a:7]:[c:8]:[c:9]:[c:10](-[O;H0;D2;+0:11]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C;D1;H3:4])(-[C;D1;H3:5])-[C;D1;H3:6]):[c:12]
83.8
[{"value": 80.0, "product": "CN(C)CCNC1=NC2=CC(=CC=C2C2=C1C(C1=CC=CC=C12)=O)OC(C(C)(C)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 83.8, "product": "CN(C)CCNC1=NC2=CC(=CC=C2C2=C1C(C1=CC=CC=C12)=O)OC(C(C)(C)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
To a solution of 6-(((dimethylamino)ethyl)amino)-3-hydroxy-7H-indeno[2,1-c]quinoline-7-on obtained in example 3 (100 mg, 0.3 mmol) in dichloromethane (10 ml) was added 4-dimethylaminopyridine (100 mg, 0.8 mmol) and pivaloyl chloride (37 μl, 0.3 mmol), and the mixture was stirred at room temperature for 3 hours. To the ...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Aromatic alcohol
Ester
null
null
c1ccc2c(c1)Cc1cnc3ccccc3c12
HCl
CN(C1=CC=NC=C1)C.ClCCl
null
3
CC(C)(C)C(=O)Cl.CN(C)CCNc1nc2cc(O)ccc2c2c1C(=O)c1ccccc1-2>CN(C1=CC=NC=C1)C.ClCCl>CN(C)CCNc1nc2cc(OC(=O)C(C)(C)C)ccc2c2c1C(=O)c1ccccc1-2
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-ce23a4c71bca4f4ba6dee847e17f8171
CN(C)CCNc1nc2cc(O)ccc2c2c1C(=O)c1ccccc1-2.O=[N+]([O-])O>>CN(C)CCNc1nc2c([N+](=O)[O-])c(O)ccc2c2c1C(=O)c1ccccc1-2
CN(C)CCNC1=NC2=CC(=CC=C2C2=C1C(C1=CC=CC=C12)=O)O.S(O)(O)(=O)=O.[N+](=O)(O)[O-]>>CN(C)CCNC1=NC2=C(C(=CC=C2C2=C1C(C1=CC=CC=C12)=O)O)[N+](=O)[O-]
[CH3:1][N:2]([CH3:3])[CH2:4][CH2:5][NH:6][c:7]1[n:8][c:9]2[cH:10][c:14]([OH:15])[cH:16][cH:17][c:18]2[c:19]2[c:20]1[C:21](=[O:22])[c:23]1[cH:24][cH:25][cH:26][cH:27][c:28]1-2.O[N+:11](=[O:12])[O-:13]>>[CH3:1][N:2]([CH3:3])[CH2:4][CH2:5][NH:6][c:7]1[n:8][c:9]2[c:10]([N+:11](=[O:12])[O-:13])[c:14]([OH:15])[cH:16][cH:17][...
CN(C)CCNc1nc2cc(O)ccc2c2c1C(=O)c1ccccc1-2.O=[N+]([O-])O
CN(C)CCNc1nc2c([N+](=O)[O-])c(O)ccc2c2c1C(=O)c1ccccc1-2
null
null
null
Functional Group Addition
Aromatic nitration with HNO3
72df91ab04c1aa0276ed1cd35e65c268b12f156077bf94b083e8543d8aab8581
ddce49825c02b8965f10c8d99e3c841d26e1f136da6037b417c09313e6d73097
O=C1c2ccccc2-c2c1cnc1ccccc21
O-[N+;H0;D3:1](-[O;-;D1;H0:2])=[O;D1;H0:3].[O;D1;H1:4]-[c:5](:[c:6]):[cH;D2;+0:7]:[c:8](:[c:9]):[#7;a:10]:[c:11]>>[O;-;D1;H0:2]-[N+;H0;D3:1](=[O;D1;H0:3])-[c;H0;D3;+0:7](:[c:5](-[O;D1;H1:4]):[c:6]):[c:8](:[c:9]):[#7;a:10]:[c:11]
52.9
[{"value": 52.9, "product": "CN(C)CCNC1=NC2=C(C(=CC=C2C2=C1C(C1=CC=CC=C12)=O)O)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}]
5
CELSIUS
2
HOUR
A mixture of 6-(((dimethylamino)ethyl)amino)-3-hydroxy-7H-indeno[2,1-c]quinoline-7-on obtained in example 3 (100 mg, 0.3 mmol), conc. sulfuric acid (1 ml) and nitric acid (1 ml) was stirred at 5° C. for 2 hours. The reaction mixture was poured into ice water, and a crystal precipitated was collected by filtration. The ...
10.6084/m9.figshare.5104873.v1
null
Nitrate
Nitro group
c1ccc2c(c1)Cc1cnc3ccccc3c12
c1ccc2c(c1)Cc1cnc3ccccc3c12
c1ccc2c(c1)Cc1cnc3ccccc3c12
HO-
null
5
2
CN(C)CCNc1nc2cc(O)ccc2c2c1C(=O)c1ccccc1-2.O=[N+]([O-])O>>CN(C)CCNc1nc2c([N+](=O)[O-])c(O)ccc2c2c1C(=O)c1ccccc1-2
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-b9d97a55e700483bba5a21fd55b4d6fd
CN(C)CCO.O=C1c2cc3c(cc2-c2c1c(Cl)nc1ccccc21)OCO3>>CN(C)CCOc1nc2ccccc2c2c1C(=O)c1cc3c(cc1-2)OCO3
[Na].CN(CCO)C.ClC1=NC2=CC=CC=C2C2=C1C(C1=CC3=C(C=C12)OCO3)=O>>CN(CCOC1=NC2=CC=CC=C2C2=C1C(C1=CC3=C(C=C12)OCO3)=O)C
[CH3:1][N:2]([CH3:3])[CH2:4][CH2:5][OH:6].Cl[c:7]1[n:8][c:9]2[cH:10][cH:11][cH:12][cH:13][c:14]2[c:15]2[c:16]1[C:17](=[O:18])[c:19]1[cH:20][c:21]3[c:22]([cH:23][c:24]1-2)[O:25][CH2:26][O:27]3>>[CH3:1][N:2]([CH3:3])[CH2:4][CH2:5][O:6][c:7]1[n:8][c:9]2[cH:10][cH:11][cH:12][cH:13][c:14]2[c:15]2[c:16]1[C:17](=[O:18])[c:19]...
CN(C)CCO.O=C1c2cc3c(cc2-c2c1c(Cl)nc1ccccc21)OCO3
CN(C)CCOc1nc2ccccc2c2c1C(=O)c1cc3c(cc1-2)OCO3
null
null
null
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
466983d8c6e1d9879bb3fee50392b4818095df00410374b9b2492c0d73b38138
a4cafa7bcd156e21cca6eaac1b32e28ec8540642a31181122e6957f3d7559631
O=C1c2cc3c(cc2-c2c1cnc1ccccc21)OCO3
Cl-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4](:[c:5])-[C:6](=[O;D1;H0:7])-[c:8].[C:9]-[C:10]-[OH;D1;+0:11]>>[C:9]-[C:10]-[O;H0;D2;+0:11]-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[c:4](:[c:5])-[C:6](=[O;D1;H0:7])-[c:8]
68.1
[{"value": 68.1, "product": "CN(CCOC1=NC2=CC=CC=C2C2=C1C(C1=CC3=C(C=C12)OCO3)=O)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 68.1, "product": "CN(CCOC1=NC2=CC=CC=C2C2=C1C(C1=CC3=C(C=C12)OCO3)=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
null
null
To a solution prepared with sodium (1.78 g, 77.4 mmol) and 2-dimethylaminoethanol (80 ml, 796 mmol) was added 6-chloro-9,10-methylenedioxy-7H-indeno[2,1-c]quinoline-7-on (8 g, 25.8 mmol) obtained in reference example 2, and the mixture was stirred with heat at 60° C. for 24 hours. The reaction mixture was poured into i...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary alcohol
Ether
c1ccc2c(c1)ncc1c2c2cc3c(cc2C1)OCO3
c1ccc2c(c1)ncc1c2c2cc3c(cc2C1)OCO3
c1ccc2c(c1)ncc1c2c2cc3c(cc2C1)OCO3
HCl
null
60
null
CN(C)CCO.O=C1c2cc3c(cc2-c2c1c(Cl)nc1ccccc21)OCO3>>CN(C)CCOc1nc2ccccc2c2c1C(=O)c1cc3c(cc1-2)OCO3
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-8b31f28fee234e13852a8ce8d1ee7421
CSc1ncc(C#N)c(O)n1.O=P(Cl)(Cl)Cl>>CSc1ncc(C#N)c(Cl)n1
C(#N)C=1C(=NC(=NC1)SC)O.P(=O)(Cl)(Cl)Cl>>ClC1=NC(=NC=C1C#N)SC
O[c:9]1[c:6]([C:7]#[N:8])[cH:5][n:4][c:3]([S:2][CH3:1])[n:11]1.O=P(Cl)(Cl)[Cl:10]>>[CH3:1][S:2][c:3]1[n:4][cH:5][c:6]([C:7]#[N:8])[c:9]([Cl:10])[n:11]1
CSc1ncc(C#N)c(O)n1.O=P(Cl)(Cl)Cl
CSc1ncc(C#N)c(Cl)n1
null
null
null
Functional Group Interconversion
Alcohol to chloride_POCl3_ortho
c34cc3a735ba90a6ebc3a31af86c6a0085713d9dcab569055caa3b8d444bb07d
e71580a8ffadb7b2717ecd7d68c1d3c0ca161ba5e6a787a49dad5a1359adc993
c1cncnc1
Cl-P(-Cl)(=O)-[Cl;H0;D1;+0:1].O-[c;H0;D3;+0:2]1:[#7;a:3]:[c:4](-[#16:5]):[#7;a:6]:[c:7]:[c:8]:1-[C:9]#[N;D1;H0:10]>>[#16:5]-[c:4]1:[#7;a:3]:[c;H0;D3;+0:2](-[Cl;H0;D1;+0:1]):[c:8](-[C:9]#[N;D1;H0:10]):[c:7]:[#7;a:6]:1
null
[]
null
null
null
null
A mixture of 5-cyano-4-hydroxy-2-methylsulfanylpyrimidine (48.33 g) from Example 1 and phosphorus oxychloride (150 mL) was heated at reflux for 3 hours. The reaction mixture was allowed to cool to room temperature, filtered, and the filtrate was concentrated to dryness under vacuum. The residue was partitioned between ...
10.6084/m9.figshare.5104873.v1
null
Aromatic alcohol
Aromatic halide
c1cncnc1
c1cncnc1
c1cncnc1
HCl
null
null
null
CSc1ncc(C#N)c(O)n1.O=P(Cl)(Cl)Cl>>CSc1ncc(C#N)c(Cl)n1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-3c865d11870445439885fc69ae3775bc
CNc1nc(NN)ncc1C#N>>CNc1nc(N=[N+]=[N-])ncc1C#N
N(=O)[O-].[Na+].C(#N)C=1C(=NC(=NC1)NN)NC.Cl>>N(=[N+]=[N-])C1=NC=C(C(=N1)NC)C#N
[CH3:1][NH:2][c:3]1[n:4][c:5]([NH:6][NH2:7])[n:9][cH:10][c:11]1[C:12]#[N:13]>>[CH3:1][NH:2][c:3]1[n:4][c:5]([N:6]=[N+:7]=[N-:8])[n:9][cH:10][c:11]1[C:12]#[N:13]
CNc1nc(NN)ncc1C#N
CNc1nc(N=[N+]=[N-])ncc1C#N
null
null
O
Functional Group Interconversion
OtherReaction
238247da1d2da37def182788bc0f9fd914e93bf24d8f65df54deba7c01d5ce90
fcfda441f91d6f59460078f0578a86bbab055471ecbff1b88b2ee65bf6892672
c1cncnc1
[NH2;D1;+0:1]-[NH;D2;+0:2]-[c:3](:[#7;a:4]:[c:5]):[#7;a:6]:[c:7]>>[N;-;D1;H0:8]=[N+;H0;D2:1]=[N;H0;D2;+0:2]-[c:3](:[#7;a:4]:[c:5]):[#7;a:6]:[c:7]
96.8
[{"value": 96.8, "product": "N(=[N+]=[N-])C1=NC=C(C(=N1)NC)C#N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
5
CELSIUS
20
MINUTE
To a cold (5° C.) solution of 5-cyano-2-hydrazino-4-methylamino-pyrimidine (21.7 g) from Example 4 in a mixture of water (260 mL) and concentrated HCl (26.5 mL) was added dropwise a solution of NaNO2 (10.03 g) in water (25 mL) with overhead mechanical stirring. A white precipitate formed and after the addition was comp...
10.6084/m9.figshare.5104873.v1
null
Hydrazine
Azide
null
null
c1cncnc1
null
O
5
0.333333
CNc1nc(NN)ncc1C#N>O>CNc1nc(N=[N+]=[N-])ncc1C#N
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-30431f184fdc4b00a734c5fabc99cc4f
CNc1nc(N=[N+]=[N-])ncc1C#N.O=CO>>CNc1nc(N)ncc1C=O
N(=[N+]=[N-])C1=NC=C(C(=N1)NC)C#N.C(=O)O.[H][H]>>NC1=NC=C(C(=N1)NC)C=O
N#[C:10][c:9]1[c:3]([NH:2][CH3:1])[n:4][c:5]([N:6]=[N+]=[N-])[n:7][cH:8]1.OC=[O:11]>>[CH3:1][NH:2][c:3]1[n:4][c:5]([NH2:6])[n:7][cH:8][c:9]1[CH:10]=[O:11]
CNc1nc(N=[N+]=[N-])ncc1C#N.O=CO
CNc1nc(N)ncc1C=O
null
[Ni].[Ni]
null
Miscellaneous
OtherReaction
3353e7bb07a95f9ddc36fda04e1ee037bcb76832d7d05908a7ce09412e4bd137
f3e2c23d9f38fc7b23dd8650cee0eab791b6ee1ce7d6cb2640cd5ee5858186e4
c1cncnc1
N#[C;H0;D2;+0:1]-[c:2]1:[c:3]:[#7;a:4]:[c:5](-[N;H0;D2;+0:6]=[N+]=[N-]):[#7;a:7]:[c:8]:1-[#7:9].O-C=[O;H0;D1;+0:10]>>[#7:9]-[c:8]1:[#7;a:7]:[c:5](-[NH2;D1;+0:6]):[#7;a:4]:[c:3]:[c:2]:1-[CH;D2;+0:1]=[O;H0;D1;+0:10]
null
[]
null
null
30
MINUTE
To a suspension of 2-azido-5-cyano-4-methylaminopyrimidine (22.24 g) from Example 5 in 400 mL of 50% aqueous formic acid was added Raney Nickel catalyst (5 g). The reaction mixture was shaken under an atmosphere of hydrogen (40.1 psi) in a Parr hydrogenation apparatus. There was a vigorous evolution of gas as the mixtu...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Azide.Nitrile
Aldehyde.Primary amine
null
null
c1cncnc1
Other
[Ni].[Ni]
null
0.5
CNc1nc(N=[N+]=[N-])ncc1C#N.O=CO>[Ni].[Ni]>CNc1nc(N)ncc1C=O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-c7d58afcdbc5402387de5b23c0166a3e
N#CCc1c(Cl)cccc1Cl.Nc1ncc(C=O)c(N)n1>>Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(N)nc2n1
C(C)OCC[O-].[Na+].[Na].NC1=NC=C(C(=N1)N)C=O.ClC1=C(C(=CC=C1)Cl)CC#N>>NC=1N=CC2=C(N1)N=C(C(=C2)C2=C(C=CC=C2Cl)Cl)N
[CH2:7]([c:8]1[c:9]([Cl:10])[cH:11][cH:12][cH:13][c:14]1[Cl:15])[C:16]#[N:17].O=[CH:6][c:5]1[cH:4][n:3][c:2]([NH2:1])[n:20][c:19]1[NH2:18]>>[NH2:1][c:2]1[n:3][cH:4][c:5]2[cH:6][c:7](-[c:8]3[c:9]([Cl:10])[cH:11][cH:12][cH:13][c:14]3[Cl:15])[c:16]([NH2:17])[n:18][c:19]2[n:20]1
N#CCc1c(Cl)cccc1Cl.Nc1ncc(C=O)c(N)n1
Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(N)nc2n1
null
null
C(C)OCCO
Aromatic Heterocycle Formation
OtherReaction
457efb65ee92bdd64de5e4c4637aa6a6f5956ef7df9875f74f905470843f8329
ee9b166152faf84f609712c2b467526aa08715073838c269f02320595214b178
c1ccc(-c2cnc3ncncc3c2)cc1
O=[CH;D2;+0:1]-[c:2]1:[c:3]:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[NH2;D1;+0:8].[Cl;D1;H0:9]-[c:10](:[c:11]):[c;H0;D3;+0:12](-[CH2;D2;+0:13]-[C;H0;D2;+0:14]#[N;H0;D1;+0:15]):[c:16](-[Cl;D1;H0:17]):[c:18]>>[Cl;D1;H0:9]-[c:10](:[c:11]):[c;H0;D3;+0:12](-[c;H0;D3;+0:13]1:[cH;D2;+0:1]:[c:2]2:[c:3]:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:2:...
null
[]
null
null
null
null
(Prepared by the method of U.S. Pat. No. 3,534,039). To a solution of sodium 2-ethoxyethoxide prepared from 0.14 g of sodium and 60 mL of 2-ethoxyethanol was added 2.07 g of 2,4-diamino-5-pyrimidinecarboxaldehyde, and 2.79 g of 2,6-dichlorophenylacetonitrile. The mixture was heated at reflux for 4 hours, allowed to coo...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Nitrile.Primary amine
Primary amine
c1cncnc1
c1cnc2ncncc2c1
c1cnc2ncncc2c1.c1ccccc1
HO-
C(C)OCCO
null
null
N#CCc1c(Cl)cccc1Cl.Nc1ncc(C=O)c(N)n1>C(C)OCCO>Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(N)nc2n1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-6e29f6338ec248b690e8a6491c1779c2
CI.Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(O)nc2n1>>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
[H-].[Na+].NC=1N=CC2=C(N1)N=C(C(=C2)C2=C(C=CC=C2Cl)Cl)O.CI>>NC=1N=CC2=C(N1)N(C(C(=C2)C2=C(C=CC=C2Cl)Cl)=O)C
I[CH3:1].[n:2]1[c:3]([OH:4])[c:5](-[c:6]2[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]2[Cl:13])[cH:14][c:15]2[cH:16][n:17][c:18]([NH2:19])[n:20][c:21]12>>[CH3:1][n:2]1[c:3](=[O:4])[c:5](-[c:6]2[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]2[Cl:13])[cH:14][c:15]2[cH:16][n:17][c:18]([NH2:19])[n:20][c:21]12
CI.Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(O)nc2n1
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
null
null
CN(C=O)C
Acylation
OtherReaction
7dd5a2fccb6323a5f77a4b63756fc3de8ac3d3fad89bb5d6740eb97207c75fcc
112bab89a832807e83a4911f32b3895489765458263eca889524c8ed19f7b9da
O=c1[nH]c2ncncc2cc1-c1ccccc1
I-[CH3;D1;+0:1].[OH;D1;+0:2]-[c;H0;D3;+0:3]1:[n;H0;D2;+0:4]:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:[c:10]:2:[c:11]:[c:12]:1-[c:13]>>[CH3;D1;+0:1]-[n;H0;D3;+0:4]1:[c:5]2:[#7;a:6]:[c:7]:[#7;a:8]:[c:9]:[c:10]:2:[c:11]:[c:12](-[c:13]):[c;H0;D3;+0:3]:1=[O;H0;D1;+0:2]
49.1
[{"value": 49.1, "product": "NC=1N=CC2=C(N1)N(C(C(=C2)C2=C(C=CC=C2Cl)Cl)=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
65
CELSIUS
3
HOUR
To a mixture of 2-amino-6-(2,6-dichlorophenyl)-pyrido[2,3-d]pyrimidin-7-ol (3.7 g) from Example 11 in dimethylformamide was added NaH (50% suspension in mineral oil, 0.64 g). The resulting slurry was heated at 65° C. for 0.5 hour until a solution formed. It was then cooled to 50° C. and a solution of methyl iodide (2.0...
10.6084/m9.figshare.5104873.v1
null
Aromatic alcohol
null
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1
HI
CN(C=O)C
65
3
CI.Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(O)nc2n1>CN(C=O)C>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-f8431548c7b24ab7baaa89a876f8af64
Cc1ccccc1-c1cc2cnc(N)nc2n(C)c1=N.O>>Cc1ccccc1-c1cc2cnc(N)nc2n(C)c1=O
CC1=C(C=CC=C1)C1=CC2=C(N=C(N=C2)N)N(C1=N)C.Cl.O>>NC=1N=CC2=C(N1)N(C(C(=C2)C2=C(C=CC=C2)C)=O)C
N=[c:19]1[c:8](-[c:7]2[c:2]([CH3:1])[cH:3][cH:4][cH:5][cH:6]2)[cH:9][c:10]2[cH:11][n:12][c:13]([NH2:14])[n:15][c:16]2[n:17]1[CH3:18].[OH2:20]>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1-[c:8]1[cH:9][c:10]2[cH:11][n:12][c:13]([NH2:14])[n:15][c:16]2[n:17]([CH3:18])[c:19]1=[O:20]
Cc1ccccc1-c1cc2cnc(N)nc2n(C)c1=N.O
Cc1ccccc1-c1cc2cnc(N)nc2n(C)c1=O
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
7e90239cfce707b5d71d7acd2c9920e6ba1c56c90bac03a2d6d5e6e8da49f59b
7a358c636daddc97c1fb4c29f378044d7eac3f01815d9966e599841f642d631a
O=c1[nH]c2ncncc2cc1-c1ccccc1
N=[c;H0;D3;+0:1]1:[#7;a:2](-[C;D1;H3:3]):[c:4]2:[#7;a:5]:[c:6]:[#7;a:7]:[c:8]:[c:9]:2:[c:10]:[c:11]:1-[c:12].[OH2;D0;+0:13]>>[C;D1;H3:3]-[#7;a:2]1:[c:4]2:[#7;a:5]:[c:6]:[#7;a:7]:[c:8]:[c:9]:2:[c:10]:[c:11](-[c:12]):[c;H0;D3;+0:1]:1=[O;H0;D1;+0:13]
null
[]
null
null
null
null
To a mixture of 6-(2-methylphenyl)-7-imino-8-methyl-7,8-dihydro-pyrido[2,3-d]pyrimidin-2-ylamine (0.30 g) from Example 8 and concentrated HCl (0.6 mL) was added water (11 mL). The reaction mixture was refluxed for 20 hours, then allowed to cool to room temperature. The white precipitate from the reaction mixture was fi...
10.6084/m9.figshare.5104873.v1
null
null
null
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1
Other
null
null
null
Cc1ccccc1-c1cc2cnc(N)nc2n(C)c1=N.O>>Cc1ccccc1-c1cc2cnc(N)nc2n(C)c1=O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-040121136d37435a8bcc1f1ef88ef22c
CC(=O)OC(C)=O.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21>>CC(=O)Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
NC=1N=CC2=C(N1)N(C(C(=C2)C2=C(C=CC=C2Cl)Cl)=O)C.C(C)(=O)OC(C)=O>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NC(C)=O)N(C1=O)C
CC(=O)O[C:2]([CH3:1])=[O:3].[NH2:4][c:5]1[n:6][cH:7][c:8]2[cH:9][c:10](-[c:11]3[c:12]([Cl:13])[cH:14][cH:15][cH:16][c:17]3[Cl:18])[c:19](=[O:20])[n:21]([CH3:22])[c:23]2[n:24]1>>[CH3:1][C:2](=[O:3])[NH:4][c:5]1[n:6][cH:7][c:8]2[cH:9][c:10](-[c:11]3[c:12]([Cl:13])[cH:14][cH:15][cH:16][c:17]3[Cl:18])[c:19](=[O:20])[n:21](...
CC(=O)OC(C)=O.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
CC(=O)Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
null
null
null
Acylation
Aminolysis of esters
87d35e51b477fc9a658a6f307eb56d84c8879182772c9dd3a42ec0d584fd2684
627cbc0550c9f51ad0105d9fcf46677e8c93bed87ee95bfe69292a82550c95b7
O=c1[nH]c2ncncc2cc1-c1ccccc1
C-C(=O)-O-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[#7;a:4]:[c:5]:[#7;a:6]:[c:7](-[NH2;D1;+0:8]):[#7;a:9]:[c:10]>>[#7;a:4]:[c:5]:[#7;a:6]:[c:7](-[NH;D2;+0:8]-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3]):[#7;a:9]:[c:10]
null
[]
25
CELSIUS
null
null
A mixture of 64.2 mg (0.20 mmol) of 2-amino-6-(2,6-dichlorophenyl)-8-methyl-pyrido[2,3-d]pyrimidin-7(8H)-one (from Example 12) and 1 mL of acetic anhydride was heated to reflux. The resulting solution was maintained at reflux for 20 minutes and concentrated at atmospheric pressure to about 0.25 mL volume. The solution ...
10.6084/m9.figshare.5104873.v1
null
Anhydride.Primary amine
Secondary amide
null
null
c1cnc2ncncc2c1.c1ccccc1
HO-
null
25
null
CC(=O)OC(C)=O.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21>>CC(=O)Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-7f755484eae34b89a6dc4eb4bf6a4b14
CNc1nc(SC)ncc1C#N.O>>CNc1nc(SC)ncc1C=O
C(#N)C=1C(=NC(=NC1)SC)NC.O>>CNC1=NC(=NC=C1C=O)SC
N#[C:11][c:10]1[c:3]([NH:2][CH3:1])[n:4][c:5]([S:6][CH3:7])[n:8][cH:9]1.[OH2:12]>>[CH3:1][NH:2][c:3]1[n:4][c:5]([S:6][CH3:7])[n:8][cH:9][c:10]1[CH:11]=[O:12]
CNc1nc(SC)ncc1C#N.O
CNc1nc(SC)ncc1C=O
null
null
C(=O)O
Heteroatom Alkylation and Arylation
OtherReaction
26082e4725cd2a7c1eb6362fc44981286c2087c015aba2f1b570103659ffb41e
e783d65987caa6ceae095ff666413e4c8d25ead96c003eb4f99d66fc68c0b0bb
c1cncnc1
N#[C;H0;D2;+0:1]-[c:2]1:[c:3]:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[#7:8].[OH2;D0;+0:9]>>[#7:8]-[c:7]1:[#7;a:6]:[c:5]:[#7;a:4]:[c:3]:[c:2]:1-[CH;D2;+0:1]=[O;H0;D1;+0:9]
null
[]
25
CELSIUS
12
HOUR
A solution of 4.00 g (0.022 mol) of 5-cyano-4-methylamino-2-methylsulfanyl-pyrimidine (from Example 3) in 150 mL of 50% aqueous formic acid was reacted with 6.0 g of water-wet Raney Nickel. The mixture was stirred at 25° C. for 12 hours. The solids were filtered and washed with 40 mL of 50% aqueous formic acid. With ic...
10.6084/m9.figshare.5104873.v1
null
Nitrile
Aldehyde
null
null
c1cncnc1
Other
C(=O)O
25
12
CNc1nc(SC)ncc1C#N.O>C(=O)O>CNc1nc(SC)ncc1C=O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-dd5613fe644d4335b125576fcb33212e
CCOC(=O)c1cnc(SC)nc1Cl.CN>>CCOC(=O)c1cnc(SC)nc1NC
CN.C(C)OC(=O)C=1C(=NC(=NC1)SC)Cl.C(C)N(CC)CC>>C(C)OC(=O)C=1C(=NC(=NC1)SC)NC
Cl[c:13]1[c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[cH:7][n:8][c:9]([S:10][CH3:11])[n:12]1.[NH2:14][CH3:15]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[cH:7][n:8][c:9]([S:10][CH3:11])[n:12][c:13]1[NH:14][CH3:15]
CCOC(=O)c1cnc(SC)nc1Cl.CN
CCOC(=O)c1cnc(SC)nc1NC
null
null
CCCCCC.O1CCCC1
Heteroatom Alkylation and Arylation
N-arylation (Buchwald-Hartwig/Ullmann-Goldberg)
c38b7155556ff28144ae37859ff6668b20d59da60c705d26b158542b6d8385da
71a04ae650defc5edd86a92f43c304e981a05f07ff76248da8d4155f3905a29d
c1cncnc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](-[#16:4]):[#7;a:5]:[c:6]:[c:7]:1-[C:8](=[O;D1;H0:9])-[#8:10]-[C:11].[C;D1;H3:12]-[NH2;D1;+0:13]>>[#16:4]-[c:3]1:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:13]-[C;D1;H3:12]):[c:7](-[C:8](=[O;D1;H0:9])-[#8:10]-[C:11]):[c:6]:[#7;a:5]:1
81
[{"value": 81.0, "product": "C(C)OC(=O)C=1C(=NC(=NC1)SC)NC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 80.4, "product": "C(C)OC(=O)C=1C(=NC(=NC1)SC)NC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
25
CELSIUS
30
MINUTE
To a solution of 4-chloro-2-methylsulfanyl-5-pyrimidinecarboxylate ethyl ester (18.66 g, 80.4 mmol) in 260 mL of tetrahydrofuran was added triethylamine (34 mL, 244 mmol), followed by 30 mL of a 40% aqueous solution of methylamine. The solution was stirred for 30 minutes at 25° C. then concentrated in vacuo and partiti...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Primary amine
Secondary amine
c1cncnc1
c1cncnc1
c1cncnc1
HCl
CCCCCC.O1CCCC1
25
0.5
CCOC(=O)c1cnc(SC)nc1Cl.CN>CCCCCC.O1CCCC1>CCOC(=O)c1cnc(SC)nc1NC
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-abfc9b5568f94a61bc5a0e552cd345d3
CCOC(=O)c1cnc(SC)nc1NC>>CNc1nc(SC)ncc1CO
C(C)OC(=O)C=1C(=NC(=NC1)SC)NC.[H-].[Al+3].[Li+].[H-].[H-].[H-]>>CNC1=NC(=NC=C1CO)SC
CCO[C:11]([c:10]1[c:3]([NH:2][CH3:1])[n:4][c:5]([S:6][CH3:7])[n:8][cH:9]1)=[O:12]>>[CH3:1][NH:2][c:3]1[n:4][c:5]([S:6][CH3:7])[n:8][cH:9][c:10]1[CH2:11][OH:12]
CCOC(=O)c1cnc(SC)nc1NC
CNc1nc(SC)ncc1CO
null
null
O1CCCC1
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
c1cncnc1
C-C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[c:3]1:[c:4]:[#7;a:5]:[c:6]:[#7;a:7]:[c:8]:1-[#7:9]>>[#7:9]-[c:8]1:[#7;a:7]:[c:6]:[#7;a:5]:[c:4]:[c:3]:1-[CH2;D2;+0:1]-[OH;D1;+0:2]
84
[{"value": 84.0, "product": "CNC1=NC(=NC=C1CO)SC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 83.6, "product": "CNC1=NC(=NC=C1CO)SC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
A solution of 4-methylamino-2-methylsulfanyl-5-pyrimidinecarboxylate ethyl ester (4.36 g, 19.3 mmol) in 60 mL of tetrahydrofuran was added dropwise to a room temperature suspension of lithium aluminum hydride (1.10 g, 29.0 mmol) in 40 mL of tetrahydrofuran. After 10 minutes the reaction was carefully quenched with 2 mL...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
c1cncnc1
HO-
O1CCCC1
null
1
CCOC(=O)c1cnc(SC)nc1NC>O1CCCC1>CNc1nc(SC)ncc1CO
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-8aa336f790624ad587b9c64aa9340829
CNc1nc(SC)ncc1CO>>CNc1nc(SC)ncc1C=O
CNC1=NC(=NC=C1CO)SC.O.O.[Cr](=O)(=O)([O-])O[Cr](=O)(=O)[O-].[Na+].[Na+].O.O.[Cr](=O)(=O)([O-])O[Cr](=O)(=O)[O-].[Na+].[Na+]>>CNC1=NC(=NC=C1C=O)SC
[CH3:1][NH:2][c:3]1[n:4][c:5]([S:6][CH3:7])[n:8][cH:9][c:10]1[CH2:11][OH:12]>>[CH3:1][NH:2][c:3]1[n:4][c:5]([S:6][CH3:7])[n:8][cH:9][c:10]1[CH:11]=[O:12]
CNc1nc(SC)ncc1CO
CNc1nc(SC)ncc1C=O
null
null
C(C)(=O)O
Oxidation
Oxidation or Dehydrogenation of Alcohols to Aldehydes and Ketones
41bfa9deea81b465c88ad21fdfb64a2e1ba29490558cf430df132cb98b4a538b
0a03c6724c1862e8f86d4a463afda55b8e067dc6cb42597b472eb7cabc03eda3
c1cncnc1
[#7:1]-[c:2]1:[#7;a:3]:[c:4]:[#7;a:5]:[c:6]:[c:7]:1-[CH2;D2;+0:8]-[OH;D1;+0:9]>>[#7:1]-[c:2]1:[#7;a:3]:[c:4]:[#7;a:5]:[c:6]:[c:7]:1-[CH;D2;+0:8]=[O;H0;D1;+0:9]
30.2
[{"value": 30.0, "product": "CNC1=NC(=NC=C1C=O)SC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 30.2, "product": "CNC1=NC(=NC=C1C=O)SC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
4-Methylamino-2-methylsulfanyl-5-pyrimidine-methanol (2.40 g, 13.0 mmol) in 7 mL of acetic acid was added to a solution of sodium dichromate-dihydrate (1.30 g, 4.4 mmol) in 6 mL of acetic acid. After 2 hours at room temperature, additional sodium dichromate-dihydrate (0.3 g, 1.0 mmol) in 1 mL of acetic acid was added. ...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Aldehyde
null
null
c1cncnc1
null
C(C)(=O)O
null
2
CNc1nc(SC)ncc1CO>C(C)(=O)O>CNc1nc(SC)ncc1C=O
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-a7d5dc196a1f4db59fce7d32888d8b45
CNc1nc(SC)ncc1C=O.N#CCc1c(Cl)cccc1Cl>>CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=N)n(C)c2n1
C(C)(=O)OCC.C([O-])([O-])=O.[K+].[K+].CNC1=NC(=NC=C1C=O)SC.ClC1=C(C(=CC=C1)Cl)CC#N.CN(C=O)C>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)SC)N(C1=N)C
O=[CH:7][c:6]1[cH:5][n:4][c:3]([S:2][CH3:1])[n:22][c:21]1[NH:19][CH3:20].[CH2:8]([c:9]1[c:10]([Cl:11])[cH:12][cH:13][cH:14][c:15]1[Cl:16])[C:17]#[N:18]>>[CH3:1][S:2][c:3]1[n:4][cH:5][c:6]2[cH:7][c:8](-[c:9]3[c:10]([Cl:11])[cH:12][cH:13][cH:14][c:15]3[Cl:16])[c:17](=[NH:18])[n:19]([CH3:20])[c:21]2[n:22]1
CNc1nc(SC)ncc1C=O.N#CCc1c(Cl)cccc1Cl
CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=N)n(C)c2n1
null
null
C(Cl)Cl
Aromatic Heterocycle Formation
OtherReaction
0563001d31884c03e15e9f4307d31ffde7ef37fabfd8267db28237eb39076249
869483589005a5aba7d1617b2e2f826aa2ded09152e8d61d0607fd18c3c9c8b9
N=c1[nH]c2ncncc2cc1-c1ccccc1
O=[CH;D2;+0:1]-[c:2]1:[c:3]:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[NH;D2;+0:8]-[C;D1;H3:9].[Cl;D1;H0:10]-[c:11](:[c:12]):[c;H0;D3;+0:13](-[CH2;D2;+0:14]-[C;H0;D2;+0:15]#[N;H0;D1;+0:16]):[c:17](-[Cl;D1;H0:18]):[c:19]>>[C;D1;H3:9]-[n;H0;D3;+0:8]1:[c:7]2:[#7;a:6]:[c:5]:[#7;a:4]:[c:3]:[c:2]:2:[cH;D2;+0:1]:[c;H0;D3;+0:14](-[c;H0;...
40
[{"value": 40.0, "product": "ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)SC)N(C1=N)C", "details": "PERCENTYIELD", "is_desired": false}]
125
CELSIUS
6
HOUR
Powdered potassium carbonate (0.8 g; 5.8 mmol) was added to a solution of 0.220 g (1.2 mmol) of the aldehyde from Example 18 and 0.235 g (1.26 mmol) (ca. 5% excess) of 2,6-dichlorophenylacetonitrile in 2.0 mL of dimethylformamide. The mixture was heated with stirring at 125° C. for 6 hours. Ethyl acetate (5 mL) was add...
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Nitrile.Secondary amine
null
c1cncnc1
c1cnc2ncncc2c1
c1cnc2ncncc2c1.c1ccccc1
HO-
C(Cl)Cl
125
6
CNc1nc(SC)ncc1C=O.N#CCc1c(Cl)cccc1Cl>C(Cl)Cl>CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=N)n(C)c2n1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-35741f9734764022a52b0d43501cf256
CCOCCOc1ncc2cc(-c3c(Cl)cccc3Cl)c(=N)n(C)c2n1>>Cl.Cn1c(=N)c(-c2c(Cl)cccc2Cl)cc2cnc(O)nc21
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)OCCOCC)N(C1=N)C>>Cl.ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)O)N(C1=N)C
CCOCC[O:20][c:19]1[n:18][cH:17][c:16]2[cH:15][c:6](-[c:7]3[c:8]([Cl:1])[cH:10][cH:11][cH:12][c:13]3[Cl:14])[c:4](=[NH:5])[n:3]([CH3:2])[c:22]2[n:21]1>>[ClH:1].[CH3:2][n:3]1[c:4](=[NH:5])[c:6](-[c:7]2[c:8]([Cl:9])[cH:10][cH:11][cH:12][c:13]2[Cl:14])[cH:15][c:16]2[cH:17][n:18][c:19]([OH:20])[n:21][c:22]12
CCOCCOc1ncc2cc(-c3c(Cl)cccc3Cl)c(=N)n(C)c2n1
Cl.Cn1c(=N)c(-c2c(Cl)cccc2Cl)cc2cnc(O)nc21
null
null
Cl
Miscellaneous
OtherReaction
b4cea5b2d239b73e5c5aee3137cdaad3b3f8aa211f3a34a1cea4e9dd11de1feb
c427c467a576ca94eabe2e08bd6347a4b9bbc0385f3c9122178b52dbe50a75a3
N=c1[nH]c2ncncc2cc1-c1ccccc1
C-C-O-C-C-[O;H0;D2;+0:1]-[c:2](:[#7;a:3]:[c:4]):[#7;a:5]:[c:6]:[#7;a:7]:[c:8]:[c:9]-[c:10](:[c:11]):[c;H0;D3;+0:12](-[Cl;H0;D1;+0:13]):[c:14]:[c:15]>>[Cl;D1;H0:16]-[c;H0;D3;+0:12](:[c:14]:[c:15]):[c:10](-[c:9]:[c:8]:[#7;a:7]:[c:6]:[#7;a:5]:[c:2](-[OH;D1;+0:1]):[#7;a:3]:[c:4]):[c:11].[ClH;D0;+0:13]
null
[]
null
null
null
null
A solution of 78.0 mg (0.20 mmol) of the ethoxyethyl ether from Example 22 in 1.0 mL of 6N hydrochloric acid was heated at reflux for 5 minutes. The solvent was removed by evaporation under reduced pressure. The remaining solid hydrochloride salt was recrystallized from ethanol-ethyl acetate to afford crystalline 6-(2,...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ether.Ether
Aromatic halide.Aromatic alcohol
c1ccccc1
c1ccccc1
c1ccccc1.c1cnc2ncncc2c1
HO-
Cl
null
null
CCOCCOc1ncc2cc(-c3c(Cl)cccc3Cl)c(=N)n(C)c2n1>Cl>Cl.Cn1c(=N)c(-c2c(Cl)cccc2Cl)cc2cnc(O)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-9cc63b0f6a514bce8d35b9f03404b410
COc1ccc(P2(=S)SP(=S)(c3ccc(OC)cc3)S2)cc1.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21>>Cn1c(=S)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
NC=1N=CC2=C(N1)N(C(C(=C2)C2=C(C=CC=C2Cl)Cl)=O)C.COC=1C=CC(=CC1)P2(=S)SP(=S)(S2)C=3C=CC(=CC3)OC>>NC=1N=CC2=C(N1)N(C(C(=C2)C2=C(C=CC=C2Cl)Cl)=S)C
COc1ccc(P2(=S)SP(c3ccc(OC)cc3)(=[S:4])S2)cc1.O=[c:3]1[n:2]([CH3:1])[c:21]2[c:15]([cH:14][c:5]1-[c:6]1[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]1[Cl:13])[cH:16][n:17][c:18]([NH2:19])[n:20]2>>[CH3:1][n:2]1[c:3](=[S:4])[c:5](-[c:6]2[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]2[Cl:13])[cH:14][c:15]2[cH:16][n:17][c:18]([NH2:19])[n:...
COc1ccc(P2(=S)SP(=S)(c3ccc(OC)cc3)S2)cc1.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
Cn1c(=S)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
null
null
N1=CC=CC=C1
Heteroatom Alkylation and Arylation
OtherReaction
cffb02ee009c6075673bb4ccc2b6ab6758ccd066ab0e544ca5420e501c92747c
6988b5bdf4783315bb3059677289ee20aff4c88fbf4684f4ee12b75839fcb0a0
S=c1[nH]c2ncncc2cc1-c1ccccc1
C-O-c1:c:c:c(-P2(=S)-S-P(=[S;H0;D1;+0:1])(-c3:c:c:c(-O-C):c:c:3)-S-2):c:c:1.O=[c;H0;D3;+0:2](:[#7;a:3](-[C;D1;H3:4]):[c:5]:[#7;a:6]):[c:7](-[c:8]):[c:9]>>[#7;a:6]:[c:5]:[#7;a:3](-[C;D1;H3:4]):[c;H0;D3;+0:2](=[S;H0;D1;+0:1]):[c:7](-[c:8]):[c:9]
null
[]
null
null
24
HOUR
A mixture of 0.321 g (1.0 mmol) of 2-amino-6-(2,6-dichlorophenyl)-8-methyl-pyrido[2,3-d]pyrimidin-7-(8H)-one from Example 12 and 0.404 g (1.0 mmol) of Lawesson's Reagent in 10 mL of pyridine was heated at reflux with stirring for 24 hours. The solvent was evaporated under reduced pressure, and the residue was triturate...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Monosulfide.Monosulfide
Thiocarbonyl
c1ccccc1.P1SPS1.c1ccccc1.c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1
Other
N1=CC=CC=C1
null
24
COc1ccc(P2(=S)SP(=S)(c3ccc(OC)cc3)S2)cc1.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21>N1=CC=CC=C1>Cn1c(=S)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-de9b6ae759eb4e73bdbda8a0c8140fe5
CC(=O)OC(C)=O.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=N)n(C)c2n1>>CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=NC(C)=O)n(C)c2n1
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)SC)N(C1=N)C.C(C)(=O)OC(C)=O>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)SC)N(C1=NC(C)=O)C
CC(=O)O[C:19]([CH3:20])=[O:21].[CH3:1][S:2][c:3]1[n:4][cH:5][c:6]2[cH:7][c:8](-[c:9]3[c:10]([Cl:11])[cH:12][cH:13][cH:14][c:15]3[Cl:16])[c:17](=[NH:18])[n:22]([CH3:23])[c:24]2[n:25]1>>[CH3:1][S:2][c:3]1[n:4][cH:5][c:6]2[cH:7][c:8](-[c:9]3[c:10]([Cl:11])[cH:12][cH:13][cH:14][c:15]3[Cl:16])[c:17](=[N:18][C:19]([CH3:20])=...
CC(=O)OC(C)=O.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=N)n(C)c2n1
CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=NC(C)=O)n(C)c2n1
null
null
CCOCC
Acylation
Aminolysis of esters
868ba94f028b30e9347f1568001d166d126ab48ad34862bd252bb72f87967edd
93289da630dbaf2d9339c4212dcd342dfbcc29df4e79a63418a0fd9f589abdc1
N=c1[nH]c2ncncc2cc1-c1ccccc1
C-C(=O)-O-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[#7;a:4]:[c:5]:[#7;a:6](-[C;D1;H3:7]):[c:8](=[NH;D1;+0:9]):[c:10]>>[#7;a:4]:[c:5]:[#7;a:6](-[C;D1;H3:7]):[c:8](=[N;H0;D2;+0:9]-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3]):[c:10]
null
[]
null
null
null
null
A mixture of 0.161 g (0.46 mmol) of 6-(2,6-dichlorophenyl)-8-methyl-2-methylsulfanyl-8H-pyrido[2,3 -d]pyrimidin-7-ylideneamine from Example 19 and 1.0 mL of acetic anhydride was heated to solution at the boiling point. After 2 minutes of reflux, the solution was concentrated to one-half volume, whereupon crystals forme...
10.6084/m9.figshare.5104873.v1
null
Anhydride
null
null
null
c1cnc2ncncc2c1.c1ccccc1
HO-
CCOCC
null
null
CC(=O)OC(C)=O.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=N)n(C)c2n1>CCOCC>CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=NC(C)=O)n(C)c2n1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-dc089cf7000c4b12a70b5ffd130e6b36
CCI.Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(O)nc2n1>>CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
NC=1N=CC2=C(N1)N=C(C(=C2)C2=C(C=CC=C2Cl)Cl)O.[H-].[Na+].C(C)I>>NC=1N=CC2=C(N1)N(C(C(=C2)C2=C(C=CC=C2Cl)Cl)=O)CC
I[CH2:2][CH3:1].[n:3]1[c:4]([OH:5])[c:6](-[c:7]2[c:8]([Cl:9])[cH:10][cH:11][cH:12][c:13]2[Cl:14])[cH:15][c:16]2[cH:17][n:18][c:19]([NH2:20])[n:21][c:22]12>>[CH3:1][CH2:2][n:3]1[c:4](=[O:5])[c:6](-[c:7]2[c:8]([Cl:9])[cH:10][cH:11][cH:12][c:13]2[Cl:14])[cH:15][c:16]2[cH:17][n:18][c:19]([NH2:20])[n:21][c:22]12
CCI.Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(O)nc2n1
CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
null
null
CN(C=O)C
Acylation
OtherReaction
d4508e77261150488c4c1380432c15a2d90e999afdd39fb804eb30619cd6fa28
1ace3814128badf62d481904cb0fc2463e51f1c5bfb35fa1f883a03bb843d915
O=c1[nH]c2ncncc2cc1-c1ccccc1
I-[CH2;D2;+0:1]-[C;D1;H3:2].[OH;D1;+0:3]-[c;H0;D3;+0:4]1:[n;H0;D2;+0:5]:[c:6]2:[#7;a:7]:[c:8]:[#7;a:9]:[c:10]:[c:11]:2:[c:12]:[c:13]:1-[c:14]>>[C;D1;H3:2]-[CH2;D2;+0:1]-[n;H0;D3;+0:5]1:[c:6]2:[#7;a:7]:[c:8]:[#7;a:9]:[c:10]:[c:11]:2:[c:12]:[c:13](-[c:14]):[c;H0;D3;+0:4]:1=[O;H0;D1;+0:3]
55.4
[{"value": 55.0, "product": "NC=1N=CC2=C(N1)N(C(C(=C2)C2=C(C=CC=C2Cl)Cl)=O)CC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 55.4, "product": "NC=1N=CC2=C(N1)N(C(C(=C2)C2=C(C=CC=C2Cl)Cl)=O)CC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
50
CELSIUS
3.5
HOUR
To a suspension of NaH (60% in mineral oil, 27 mg) in 5 mL of dimethylformamide was added 2-amino-6-(2,6-dichlorophenyl)-pyrido[2,3-d]pyrimidin-7(8H)-one (172 mg, 0.56 mmol) from Example 11. The mixture was heated at 50° C. for 1 hour resulting in a clear solution. Ethyl iodide (60 μL, 0.75 mmol) was added, and the sol...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic alcohol
null
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1
HI
CN(C=O)C
50
3.5
CCI.Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(O)nc2n1>CN(C=O)C>CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-e91dd296e2224593a86fc92fbc509e8b
CCCI.Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(O)nc2n1>>CCCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
NC=1N=CC2=C(N1)N=C(C(=C2)C2=C(C=CC=C2Cl)Cl)O.[H-].[Na+].ICCC>>NC=1N=CC2=C(N1)N(C(C(=C2)C2=C(C=CC=C2Cl)Cl)=O)CCC
I[CH2:3][CH2:2][CH3:1].[n:4]1[c:5]([OH:6])[c:7](-[c:8]2[c:9]([Cl:10])[cH:11][cH:12][cH:13][c:14]2[Cl:15])[cH:16][c:17]2[cH:18][n:19][c:20]([NH2:21])[n:22][c:23]12>>[CH3:1][CH2:2][CH2:3][n:4]1[c:5](=[O:6])[c:7](-[c:8]2[c:9]([Cl:10])[cH:11][cH:12][cH:13][c:14]2[Cl:15])[cH:16][c:17]2[cH:18][n:19][c:20]([NH2:21])[n:22][c:2...
CCCI.Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(O)nc2n1
CCCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
null
null
CN(C=O)C
Acylation
OtherReaction
d4508e77261150488c4c1380432c15a2d90e999afdd39fb804eb30619cd6fa28
1ace3814128badf62d481904cb0fc2463e51f1c5bfb35fa1f883a03bb843d915
O=c1[nH]c2ncncc2cc1-c1ccccc1
I-[CH2;D2;+0:1]-[C:2]-[C;D1;H3:3].[OH;D1;+0:4]-[c;H0;D3;+0:5]1:[n;H0;D2;+0:6]:[c:7]2:[#7;a:8]:[c:9]:[#7;a:10]:[c:11]:[c:12]:2:[c:13]:[c:14]:1-[c:15]>>[C;D1;H3:3]-[C:2]-[CH2;D2;+0:1]-[n;H0;D3;+0:6]1:[c:7]2:[#7;a:8]:[c:9]:[#7;a:10]:[c:11]:[c:12]:2:[c:13]:[c:14](-[c:15]):[c;H0;D3;+0:5]:1=[O;H0;D1;+0:4]
68
[{"value": 68.0, "product": "NC=1N=CC2=C(N1)N(C(C(=C2)C2=C(C=CC=C2Cl)Cl)=O)CCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 68.0, "product": "NC=1N=CC2=C(N1)N(C(C(=C2)C2=C(C=CC=C2Cl)Cl)=O)CCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
50
CELSIUS
10
MINUTE
To a suspension of NaH (60% in mineral oil, 31 mg) in 6 mL of dimethylformamide was added 2-amino-6-(2,6-dichlorophenyl)-pyrido[2,3-d]pyrimidin-7(8H)-one from Example 11 (205 mg, 0.67 mmol). The mixture was heated at 50° C. for 1 hour resulting in a clear solution. 1-Iodopropane (100 μL, 1.03 mmol) was added, and the s...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic alcohol
null
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1
HI
CN(C=O)C
50
0.166667
CCCI.Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(O)nc2n1>CN(C=O)C>CCCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-01a5e0a168094896bccae2b3b8ee6758
CCCCI.Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)[nH]c2n1>>CCCCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
NC=1N=CC2=C(N1)NC(C(=C2)C2=C(C=CC=C2Cl)Cl)=O.[H-].[Na+].ICCCC>>NC=1N=CC2=C(N1)N(C(C(=C2)C2=C(C=CC=C2Cl)Cl)=O)CCCC
I[CH2:4][CH2:3][CH2:2][CH3:1].[nH:5]1[c:6](=[O:7])[c:8](-[c:9]2[c:10]([Cl:11])[cH:12][cH:13][cH:14][c:15]2[Cl:16])[cH:17][c:18]2[cH:19][n:20][c:21]([NH2:22])[n:23][c:24]12>>[CH3:1][CH2:2][CH2:3][CH2:4][n:5]1[c:6](=[O:7])[c:8](-[c:9]2[c:10]([Cl:11])[cH:12][cH:13][cH:14][c:15]2[Cl:16])[cH:17][c:18]2[cH:19][n:20][c:21]([N...
CCCCI.Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)[nH]c2n1
CCCCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
c0bd97f4a1ce12437e73bb376c2b79161100c8750c084a20105c044989ac3551
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
O=c1[nH]c2ncncc2cc1-c1ccccc1
I-[CH2;D2;+0:1]-[C:2]-[C:3].[O;D1;H0:4]=[c:5](:[c:6]):[nH;D2;+0:7]:[c:8]1:[#7;a:9]:[c:10]:[#7;a:11]:[c:12]:[c:13]:1>>[C:3]-[C:2]-[CH2;D2;+0:1]-[n;H0;D3;+0:7](:[c:8]1:[#7;a:9]:[c:10]:[#7;a:11]:[c:12]:[c:13]:1):[c:5](=[O;D1;H0:4]):[c:6]
64
[{"value": 64.0, "product": "NC=1N=CC2=C(N1)N(C(C(=C2)C2=C(C=CC=C2Cl)Cl)=O)CCCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 63.4, "product": "NC=1N=CC2=C(N1)N(C(C(=C2)C2=C(C=CC=C2Cl)Cl)=O)CCCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
50
CELSIUS
30
MINUTE
To a suspension of NaH (60% in mineral oil, 34 mg) in 6 mL of dimethylformamide was added 2-amino-6-(2,6-dichlorophenyl)-pyrido[2,3-d]pyrimidin-7(8H)-one (202 mg, 0.66 mmol). The mixture was heated to 50° C., resulting in a clear solution. 1-Iodobutane (105 μL, 0.92 mmol) was added, and the solution was stirred at 50° ...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1
HI
CN(C=O)C
50
0.5
CCCCI.Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)[nH]c2n1>CN(C=O)C>CCCCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-398313438a35477a99dae3e5237c331e
CC(C)CI.Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)[nH]c2n1>>CC(C)Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
ICC(C)C.[H-].[Na+].NC=1N=CC2=C(N1)NC(C(=C2)C2=C(C=CC=C2Cl)Cl)=O.ICC(C)C>>NC=1N=CC2=C(N1)N(C(C(=C2)C2=C(C=CC=C2Cl)Cl)=O)CC(C)C
I[CH2:4][CH:2]([CH3:1])[CH3:3].[nH:5]1[c:6](=[O:7])[c:8](-[c:9]2[c:10]([Cl:11])[cH:12][cH:13][cH:14][c:15]2[Cl:16])[cH:17][c:18]2[cH:19][n:20][c:21]([NH2:22])[n:23][c:24]12>>[CH3:1][CH:2]([CH3:3])[CH2:4][n:5]1[c:6](=[O:7])[c:8](-[c:9]2[c:10]([Cl:11])[cH:12][cH:13][cH:14][c:15]2[Cl:16])[cH:17][c:18]2[cH:19][n:20][c:21](...
CC(C)CI.Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)[nH]c2n1
CC(C)Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
c0bd97f4a1ce12437e73bb376c2b79161100c8750c084a20105c044989ac3551
2e1e5fd9557b69cb528f6b2ffd179c67ef24ecb1a2c3994e1cdf0efe7ae19e9c
O=c1[nH]c2ncncc2cc1-c1ccccc1
I-[CH2;D2;+0:1]-[C:2](-[C;D1;H3:3])-[C;D1;H3:4].[O;D1;H0:5]=[c:6](:[c:7]):[nH;D2;+0:8]:[c:9]1:[#7;a:10]:[c:11]:[#7;a:12]:[c:13]:[c:14]:1>>[C;D1;H3:3]-[C:2](-[C;D1;H3:4])-[CH2;D2;+0:1]-[n;H0;D3;+0:8](:[c:9]1:[#7;a:10]:[c:11]:[#7;a:12]:[c:13]:[c:14]:1):[c:6](=[O;D1;H0:5]):[c:7]
51
[{"value": 51.0, "product": "NC=1N=CC2=C(N1)N(C(C(=C2)C2=C(C=CC=C2Cl)Cl)=O)CC(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 50.5, "product": "NC=1N=CC2=C(N1)N(C(C(=C2)C2=C(C=CC=C2Cl)Cl)=O)CC(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
30
MINUTE
To a suspension of NaH (60% in mineral oil, 36 mg) in 8 mL of dimethylformamide was added 2-amino-6-(2,6-dichlorophenyl)-pyrido[2,3-d]pyrimidin-7(8H)-one (205 mg, 0.67 mmol). The mixture was heated at 60° C. for 20 minutes resulting in a clear solution. 1-Iodo-2-methylpropane (110 μL, 0.94 mmol) was added, and the solu...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1
HI
CN(C=O)C
60
0.5
CC(C)CI.Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)[nH]c2n1>CN(C=O)C>CC(C)Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-db033153fe46420cb6ff2af2382ca19e
COC(=O)CCl.Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)[nH]c2n1>>COC(=O)Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
NC=1N=CC2=C(N1)NC(C(=C2)C2=C(C=CC=C2Cl)Cl)=O.[H-].[Na+].ClCC(=O)OC>>COC(CN1C(C(=CC2=C1N=C(N=C2)N)C2=C(C=CC=C2Cl)Cl)=O)=O
Cl[CH2:5][C:3]([O:2][CH3:1])=[O:4].[nH:6]1[c:7](=[O:8])[c:9](-[c:10]2[c:11]([Cl:12])[cH:13][cH:14][cH:15][c:16]2[Cl:17])[cH:18][c:19]2[cH:20][n:21][c:22]([NH2:23])[n:24][c:25]12>>[CH3:1][O:2][C:3](=[O:4])[CH2:5][n:6]1[c:7](=[O:8])[c:9](-[c:10]2[c:11]([Cl:12])[cH:13][cH:14][cH:15][c:16]2[Cl:17])[cH:18][c:19]2[cH:20][n:2...
COC(=O)CCl.Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)[nH]c2n1
COC(=O)Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
fd5ba1af7389d33cca767aae97db8ad46db379d13a808cd30e0289a97675ed04
6007d70cc3173f3039a472489995dad2781e8d749be1f1aa209b0bf2f190a4b4
O=c1[nH]c2ncncc2cc1-c1ccccc1
Cl-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#8:4]-[C;D1;H3:5].[O;D1;H0:6]=[c:7](:[c:8]):[nH;D2;+0:9]:[c:10]1:[#7;a:11]:[c:12]:[#7;a:13]:[c:14]:[c:15]:1>>[C;D1;H3:5]-[#8:4]-[C:2](=[O;D1;H0:3])-[CH2;D2;+0:1]-[n;H0;D3;+0:9](:[c:10]1:[#7;a:11]:[c:12]:[#7;a:13]:[c:14]:[c:15]:1):[c:7](=[O;D1;H0:6]):[c:8]
61
[{"value": 61.0, "product": "COC(CN1C(C(=CC2=C1N=C(N=C2)N)C2=C(C=CC=C2Cl)Cl)=O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 60.7, "product": "COC(CN1C(C(=CC2=C1N=C(N=C2)N)C2=C(C=CC=C2Cl)Cl)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
50
CELSIUS
null
null
To a suspension of NaH (60% in mineral oil, 38 mg) in 6 mL of dimethylformamide was added 2-amino-6-(2,6-dichlorophenyl)-pyrido[2,3-d]pyrimidin-7(8H)-one (203 mg, 0.66 mmol). The mixture was heated at 50° C. for 40 minutes resulting in a clear solution. Methyl chloroacetate (90 μL, 1.03 mmol) was added, and the solutio...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester
Ester
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1
HCl
CN(C=O)C
50
null
COC(=O)CCl.Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)[nH]c2n1>CN(C=O)C>COC(=O)Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-16c20da4564840b98de831447344a71e
CC(C)(C)OC(=O)CBr.Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)[nH]c2n1>>CC(C)(C)OC(=O)Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
NC=1N=CC2=C(N1)NC(C(=C2)C2=C(C=CC=C2Cl)Cl)=O.[H-].[Na+].BrCC(=O)OC(C)(C)C>>C(C)(C)(C)OC(CN1C(C(=CC2=C1N=C(N=C2)N)C2=C(C=CC=C2Cl)Cl)=O)=O
Br[CH2:8][C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7].[nH:9]1[c:10](=[O:11])[c:12](-[c:13]2[c:14]([Cl:15])[cH:16][cH:17][cH:18][c:19]2[Cl:20])[cH:21][c:22]2[cH:23][n:24][c:25]([NH2:26])[n:27][c:28]12>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][n:9]1[c:10](=[O:11])[c:12](-[c:13]2[c:14]([Cl:15])[cH:16][c...
CC(C)(C)OC(=O)CBr.Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)[nH]c2n1
CC(C)(C)OC(=O)Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
Boc amine protection (ethyl Boc)
fd5ba1af7389d33cca767aae97db8ad46db379d13a808cd30e0289a97675ed04
6007d70cc3173f3039a472489995dad2781e8d749be1f1aa209b0bf2f190a4b4
O=c1[nH]c2ncncc2cc1-c1ccccc1
Br-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#8:4]-[C:5](-[C;D1;H3:6])(-[C;D1;H3:7])-[C;D1;H3:8].[O;D1;H0:9]=[c:10](:[c:11]):[nH;D2;+0:12]:[c:13]1:[#7;a:14]:[c:15]:[#7;a:16]:[c:17]:[c:18]:1>>[C;D1;H3:6]-[C:5](-[C;D1;H3:7])(-[C;D1;H3:8])-[#8:4]-[C:2](=[O;D1;H0:3])-[CH2;D2;+0:1]-[n;H0;D3;+0:12](:[c:10](=[O;D1;H0:9]):[c:11]):[c:...
30.1
[{"value": 30.0, "product": "C(C)(C)(C)OC(CN1C(C(=CC2=C1N=C(N=C2)N)C2=C(C=CC=C2Cl)Cl)=O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 30.1, "product": "C(C)(C)(C)OC(CN1C(C(=CC2=C1N=C(N=C2)N)C2=C(C=CC=C2Cl)Cl)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
50
CELSIUS
null
null
To a suspension of NaH (60% in mineral oil, 67 mg) in 10 mL of dimethylformamide was added 2-amino-6-(2,6-dichlorophenyl)-pyrido[2,3-d]pyrimidin-7(8H)-one (398 mg, 1.30 mmol). The mixture was heated at 45° C. to 55° C. for 40 minutes resulting in a clear solution. Tert-butyl bromoacetate (250 μL, 1.69 mmol) was added, ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester
Ester
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1
HBr
CN(C=O)C
50
null
CC(C)(C)OC(=O)CBr.Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)[nH]c2n1>CN(C=O)C>CC(C)(C)OC(=O)Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(N)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-bfb87e53646f4c08bf6331ebf2a578a0
CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1.O=C(OO)c1cccc(Cl)c1>>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21
ClC1=CC(=CC=C1)C(=O)OO.ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)SC)N(C1=O)C.CS(=O)C>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)S(=O)(=O)C)N(C1=O)C
[CH3:1][n:2]1[c:3](=[O:4])[c:5](-[c:6]2[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]2[Cl:13])[cH:14][c:15]2[cH:16][n:17][c:18]([S:19][CH3:20])[n:23][c:24]12.Clc1cccc(C(O[OH:22])=[O:21])c1>>[CH3:1][n:2]1[c:3](=[O:4])[c:5](-[c:6]2[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]2[Cl:13])[cH:14][c:15]2[cH:16][n:17][c:18]([S:19]([CH3:20])...
CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1.O=C(OO)c1cccc(Cl)c1
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21
null
null
C(Cl)(Cl)Cl
Oxidation
OtherReaction
84855dd3f46d7f633669ce7b0a2d1343353729d5975dd53fd20abc6eb43ece69
dc6f43112eef310adb122ebf81e1733b34eff292ed27058fb45445842d61d3da
O=c1[nH]c2ncncc2cc1-c1ccccc1
Cl-c1:c:c:c:c(-C(=[O;H0;D1;+0:1])-O-[OH;D1;+0:2]):c:1.[#7;a:3]:[c:4]:[#7;a:5]:[c:6](-[S;H0;D2;+0:7]-[C;D1;H3:8]):[#7;a:9]:[c:10]>>[#7;a:3]:[c:4]:[#7;a:5]:[c:6](-[S;H0;D4;+0:7](-[C;D1;H3:8])(=[O;H0;D1;+0:1])=[O;H0;D1;+0:2]):[#7;a:9]:[c:10]
null
[]
null
null
8
HOUR
A quantity of 0.346 g (1.00 mmol) of 50% to 60% m-chloroperbenzoic acid (assuming 50% peracid was present) was added at 25° C. to a stirred solution of 0.165 g (0.47 mmol) of 6-(2,6-dichlorophenyl)-8-methyl-2-methylsulfanyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 37 in 15 mL of chloroform, and the solution was stirr...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Peroxide.Monosulfide
Sulfone
c1ccccc1
null
c1ccccc1.c1cnc2ncncc2c1
HCl
C(Cl)(Cl)Cl
null
8
CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1.O=C(OO)c1cccc(Cl)c1>C(Cl)(Cl)Cl>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-a1fc3fad89df44fb9dcbd57241fd99a3
CN.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1>>CNc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)SC)N(C1=O)C.CN>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NC)N(C1=O)C
[CH3:1][NH2:2].CS[c:3]1[n:4][cH:5][c:6]2[cH:7][c:8](-[c:9]3[c:10]([Cl:11])[cH:12][cH:13][cH:14][c:15]3[Cl:16])[c:17](=[O:18])[n:19]([CH3:20])[c:21]2[n:22]1>>[CH3:1][NH:2][c:3]1[n:4][cH:5][c:6]2[cH:7][c:8](-[c:9]3[c:10]([Cl:11])[cH:12][cH:13][cH:14][c:15]3[Cl:16])[c:17](=[O:18])[n:19]([CH3:20])[c:21]2[n:22]1
CN.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
CNc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
OtherReaction
df9d6a54bbeb74919f9913aad742e0b7c3ffefcaa8d2bb485e4914ba80c410ee
88e0224d19b2dce8f9987d52554afb32090d36ff7ee19e89dc5bf66d30974ec4
O=c1[nH]c2ncncc2cc1-c1ccccc1
C-S-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](:[c:4]:[c:5]:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[C;D1;H3:10]-[NH2;D1;+0:11]>>[C;D1;H3:10]-[NH;D2;+0:11]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](:[c:4]:[c:5]:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9]
null
[]
null
null
10
MINUTE
A quantity of 0.165 g (0.47 mmol) of 6-(2,6-dichlorophenyl)-8-methyl-2-methylsulfanyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 37 was placed in a pressure tube with a magnetic stirring bar. The tube was cooled in a dry ice-acetone bath and ca. 3 mL of monomethylamine gas was condensed in the tube. Dimethylformamide (...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Monosulfide
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1cnc2ncncc2c1.c1ccccc1
Other
CN(C=O)C
null
0.166667
CN.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1>CN(C=O)C>CNc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-3649f27493174d968301ce7cf9e817e4
CNC.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1>>CN(C)c1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)SC)N(C1=O)C.CNC>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)N(C)C)N(C1=O)C
[CH3:1][NH:2][CH3:3].CS[c:4]1[n:5][cH:6][c:7]2[cH:8][c:9](-[c:10]3[c:11]([Cl:12])[cH:13][cH:14][cH:15][c:16]3[Cl:17])[c:18](=[O:19])[n:20]([CH3:21])[c:22]2[n:23]1>>[CH3:1][N:2]([CH3:3])[c:4]1[n:5][cH:6][c:7]2[cH:8][c:9](-[c:10]3[c:11]([Cl:12])[cH:13][cH:14][cH:15][c:16]3[Cl:17])[c:18](=[O:19])[n:20]([CH3:21])[c:22]2[n:...
CNC.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
CN(C)c1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
b04bf65d5ddea11036a7e6dd1f319b06acbc4399e4bf7e6a83cd4e2648a53efe
f5aa33108984aad43441754644c214239e577e2035dc027b4aa13ab85821a21b
O=c1[nH]c2ncncc2cc1-c1ccccc1
C-S-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](:[c:4]:[c:5]:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[C;D1;H3:10]-[NH;D2;+0:11]-[C;D1;H3:12]>>[C;D1;H3:10]-[N;H0;D3;+0:11](-[C;D1;H3:12])-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](:[c:4]:[c:5]:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9]
null
[]
null
null
null
null
This compound was prepared by a procedure similar to that described in Example 40 starting with 6-(2,6-dichlorophenyl)-8-methyl-2-methylsulfanyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 37 and dimethylamine gas; mp 256°-258° C. Conditions: See reaction.notes.procedure_details. Workup: This compound was prepared by a ...
10.6084/m9.figshare.5104873.v1
null
Secondary amine.Monosulfide
Tertiary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1cnc2ncncc2c1.c1ccccc1
Other
null
null
null
CNC.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1>>CN(C)c1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-32eed9b20fbe4a80a60b8ae09427c623
CCN.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1>>CCNc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)SC)N(C1=O)C.C(C)N>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NCC)N(C1=O)C
[CH3:1][CH2:2][NH2:3].CS[c:4]1[n:5][cH:6][c:7]2[cH:8][c:9](-[c:10]3[c:11]([Cl:12])[cH:13][cH:14][cH:15][c:16]3[Cl:17])[c:18](=[O:19])[n:20]([CH3:21])[c:22]2[n:23]1>>[CH3:1][CH2:2][NH:3][c:4]1[n:5][cH:6][c:7]2[cH:8][c:9](-[c:10]3[c:11]([Cl:12])[cH:13][cH:14][cH:15][c:16]3[Cl:17])[c:18](=[O:19])[n:20]([CH3:21])[c:22]2[n:...
CCN.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
CCNc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
df9d6a54bbeb74919f9913aad742e0b7c3ffefcaa8d2bb485e4914ba80c410ee
88e0224d19b2dce8f9987d52554afb32090d36ff7ee19e89dc5bf66d30974ec4
O=c1[nH]c2ncncc2cc1-c1ccccc1
C-S-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](:[c:4]:[c:5]:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[C;D1;H3:10]-[C:11]-[NH2;D1;+0:12]>>[C;D1;H3:10]-[C:11]-[NH;D2;+0:12]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](:[c:4]:[c:5]:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9]
null
[]
null
null
null
null
This compound was prepared by a procedure similar to that described in Example 40 starting with 6-(2,6-dichlorophenyl)-8-methyl-2-methylsulfanyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 37 and ethylamine gas; mp 180°-182° C. Conditions: See reaction.notes.procedure_details. Workup: This compound was prepared by a pro...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Monosulfide
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1cnc2ncncc2c1.c1ccccc1
Other
null
null
null
CCN.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1>>CCNc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-d04022b22bcd4100a137a9c7f735c157
CC(C)N.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1>>CC(C)Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)SC)N(C1=O)C.C(C)(C)N>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NC(C)C)N(C1=O)C
[CH3:1][CH:2]([CH3:3])[NH2:4].CS[c:5]1[n:6][cH:7][c:8]2[cH:9][c:10](-[c:11]3[c:12]([Cl:13])[cH:14][cH:15][cH:16][c:17]3[Cl:18])[c:19](=[O:20])[n:21]([CH3:22])[c:23]2[n:24]1>>[CH3:1][CH:2]([CH3:3])[NH:4][c:5]1[n:6][cH:7][c:8]2[cH:9][c:10](-[c:11]3[c:12]([Cl:13])[cH:14][cH:15][cH:16][c:17]3[Cl:18])[c:19](=[O:20])[n:21]([...
CC(C)N.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
CC(C)Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
df9d6a54bbeb74919f9913aad742e0b7c3ffefcaa8d2bb485e4914ba80c410ee
88e0224d19b2dce8f9987d52554afb32090d36ff7ee19e89dc5bf66d30974ec4
O=c1[nH]c2ncncc2cc1-c1ccccc1
C-S-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](:[c:4]:[c:5]:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[C;D1;H3:10]-[C:11](-[C;D1;H3:12])-[NH2;D1;+0:13]>>[C;D1;H3:10]-[C:11](-[C;D1;H3:12])-[NH;D2;+0:13]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](:[c:4]:[c:5]:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9]
null
[]
null
null
null
null
This compound was prepared by a procedure similar to that described in Example 40 starting with 6-(2,6-dichlorophenyl)-8-methyl-2-methylsulfanyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 37 and isopropylamine; mp 194°-196° C. Conditions: See reaction.notes.procedure_details. Workup: This compound was prepared by a pro...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Monosulfide
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1cnc2ncncc2c1.c1ccccc1
Other
null
null
null
CC(C)N.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1>>CC(C)Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-a8f31c3f69e44f889459e4fbf80bb158
CCCCN.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1>>CCCCNN1C=c2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2=NC1
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)SC)N(C1=O)C.C(CCC)N>>C(CCC)NN1CN=C2C(=C1)C=C(C(N2C)=O)C2=C(C=CC=C2Cl)Cl
[CH3:1][CH2:2][CH2:3][CH2:4][NH2:5].CS[c:25]1[n:6][cH:7][c:8]2[cH:9][c:10](-[c:11]3[c:12]([Cl:13])[cH:14][cH:15][cH:16][c:17]3[Cl:18])[c:19](=[O:20])[n:21]([CH3:22])[c:23]2[n:24]1>>[CH3:1][CH2:2][CH2:3][CH2:4][NH:5][N:6]1[CH:7]=[c:8]2[cH:9][c:10](-[c:11]3[c:12]([Cl:13])[cH:14][cH:15][cH:16][c:17]3[Cl:18])[c:19](=[O:20]...
CCCCN.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
CCCCNN1C=c2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2=NC1
null
null
CN(C=O)C
Miscellaneous
OtherReaction
43f5647777f5edceda750ecd7279b6936f64c6fee7f4496ecb94ddf45531c6e6
95c7086dc5e33844e8536f4de4a4643f8c4c6db67b746c1239865f1497b14f4e
O=c1[nH]c2c(cc1-c1ccccc1)=CNCN=2
C-S-[c;H0;D3;+0:1]1:[n;H0;D2;+0:2]:[c;H0;D3;+0:3]2:[#7;a:4](-[C;D1;H3:5]):[c:6]:[c:7]:[c:8]:[c;H0;D3;+0:9]:2:[cH;D2;+0:10]:[n;H0;D2;+0:11]:1.[C:12]-[C:13]-[NH2;D1;+0:14]>>[C:12]-[C:13]-[NH;D2;+0:14]-[N;H0;D3;+0:11]1-[CH2;D2;+0:1]-[N;H0;D2;+0:2]=[c;H0;D3;+0:3]2:[#7;a:4](-[C;D1;H3:5]):[c:6]:[c:7]:[c:8]:[c;H0;D3;+0:9]:2=[...
null
[]
110
CELSIUS
1
HOUR
A mixture of 0.177 g (0.50 mmol) of 6-(2,6-dichlorophenyl)-8-methyl-2-methylsulfanyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 37, 10 mL of n-butylamine and 1.0 mL of dimethylformamide was heated with stirring to reflux (110° C. oil bath). After 1 hour, solution was complete. After 20 hours reflux, the excess amine an...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Monosulfide
Hydrazine
c1cnc2ncncc2c1
C1=c2cccnc2=NC[NH]1
C1=c2cccnc2=NC[NH]1.c1ccccc1
Other
CN(C=O)C
110
1
CCCCN.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1>CN(C=O)C>CCCCNN1C=c2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2=NC1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-25e5f36c73a5443aa2d8d2b4bbb40382
CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1.NCc1ccccc1>>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(NCc3ccccc3)nc21
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)SC)N(C1=O)C.C(C1=CC=CC=C1)N>>C(C1=CC=CC=C1)NC=1N=CC2=C(N1)N(C(C(=C2)C2=C(C=CC=C2Cl)Cl)=O)C
CS[c:18]1[n:17][cH:16][c:15]2[cH:14][c:5](-[c:6]3[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]3[Cl:13])[c:3](=[O:4])[n:2]([CH3:1])[c:28]2[n:27]1.[NH2:19][CH2:20][c:21]1[cH:22][cH:23][cH:24][cH:25][cH:26]1>>[CH3:1][n:2]1[c:3](=[O:4])[c:5](-[c:6]2[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]2[Cl:13])[cH:14][c:15]2[cH:16][n:17][c:18]...
CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1.NCc1ccccc1
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(NCc3ccccc3)nc21
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
OtherReaction
df9d6a54bbeb74919f9913aad742e0b7c3ffefcaa8d2bb485e4914ba80c410ee
88e0224d19b2dce8f9987d52554afb32090d36ff7ee19e89dc5bf66d30974ec4
O=c1[nH]c2nc(NCc3ccccc3)ncc2cc1-c1ccccc1
C-S-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[NH2;D1;+0:10]-[C:11]-[c:12]>>[C;D1;H3:8]-[#7;a:7](:[c:9]):[c:5]1:[#7;a:6]:[c;H0;D3;+0:1](-[NH;D2;+0:10]-[C:11]-[c:12]):[#7;a:2]:[c:3]:[c:4]:1
47.6
[{"value": 47.6, "product": "C(C1=CC=CC=C1)NC=1N=CC2=C(N1)N(C(C(=C2)C2=C(C=CC=C2Cl)Cl)=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
120
CELSIUS
5
MINUTE
A mixture of 0.165 g (0.47 mmol) of 6-(2,6-dichlorophenyl)-8-methyl-2-methylsulfanyl-8H-pyrido-[2,3-d]pyrimidin-7-one of Example 37, 0.50 g (4.70 mmol) of benzylamine and 0.5 mL of dimethylformamide was heated with stirring in a 120° C. oil bath. After 5 minutes, solution was complete. After 5 hours, the excess amine a...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Monosulfide
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1.c1ccccc1
Other
CN(C=O)C
120
0.083333
CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1.NCc1ccccc1>CN(C=O)C>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(NCc3ccccc3)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-ed41f375aaff41018a80d7b0ecb415a0
CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1.NCCCN1CCOCC1>>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(NCCCN3CCOCC3)nc21
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)SC)N(C1=O)C.NCCCN1CCOCC1>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NCCCN2CCOCC2)N(C1=O)C
CS[c:18]1[n:17][cH:16][c:15]2[cH:14][c:5](-[c:6]3[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]3[Cl:13])[c:3](=[O:4])[n:2]([CH3:1])[c:30]2[n:29]1.[NH2:19][CH2:20][CH2:21][CH2:22][N:23]1[CH2:24][CH2:25][O:26][CH2:27][CH2:28]1>>[CH3:1][n:2]1[c:3](=[O:4])[c:5](-[c:6]2[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]2[Cl:13])[cH:14][c:15]2...
CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1.NCCCN1CCOCC1
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(NCCCN3CCOCC3)nc21
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
OtherReaction
df9d6a54bbeb74919f9913aad742e0b7c3ffefcaa8d2bb485e4914ba80c410ee
88e0224d19b2dce8f9987d52554afb32090d36ff7ee19e89dc5bf66d30974ec4
O=c1[nH]c2nc(NCCCN3CCOCC3)ncc2cc1-c1ccccc1
C-S-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[C:10]-[C:11]-[NH2;D1;+0:12]>>[C:10]-[C:11]-[NH;D2;+0:12]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9]
null
[]
125
CELSIUS
2
MINUTE
A mixture of 0.165 g (0.47 mmol) of 6-(2,6-dichlorophenyl)-8-methyl-2-methylsulfanyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 37, 1.00 g (6.90 mmol) of N-(3-aminopropyl)morpholine and 0.5 mL of dimethylformamide was heated with stirring in a 125° C. oil bath. After 2 minutes, solution was complete. After 1.5 hours, t...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Monosulfide
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1.C1COCC[NH]1
Other
CN(C=O)C
125
0.033333
CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1.NCCCN1CCOCC1>CN(C=O)C>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(NCCCN3CCOCC3)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-4065ebd450dd42b9b396a7e3dbade98c
CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1.NCc1ccccn1>>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(NCc3ccccn3)nc21
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)SC)N(C1=O)C.NCC1=NC=CC=C1>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NCC2=NC=CC=C2)N(C1=O)C
CS[c:18]1[n:17][cH:16][c:15]2[cH:14][c:5](-[c:6]3[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]3[Cl:13])[c:3](=[O:4])[n:2]([CH3:1])[c:28]2[n:27]1.[NH2:19][CH2:20][c:21]1[cH:22][cH:23][cH:24][cH:25][n:26]1>>[CH3:1][n:2]1[c:3](=[O:4])[c:5](-[c:6]2[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]2[Cl:13])[cH:14][c:15]2[cH:16][n:17][c:18](...
CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1.NCc1ccccn1
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(NCc3ccccn3)nc21
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
OtherReaction
df9d6a54bbeb74919f9913aad742e0b7c3ffefcaa8d2bb485e4914ba80c410ee
88e0224d19b2dce8f9987d52554afb32090d36ff7ee19e89dc5bf66d30974ec4
O=c1[nH]c2nc(NCc3ccccn3)ncc2cc1-c1ccccc1
C-S-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[#7;a:10]:[c:11]-[C:12]-[NH2;D1;+0:13]>>[#7;a:10]:[c:11]-[C:12]-[NH;D2;+0:13]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9]
38.7
[{"value": 38.7, "product": "ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NCC2=NC=CC=C2)N(C1=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
130
CELSIUS
2
MINUTE
A mixture of 0.165 g (0.47 mmol) of 6-(2,6-dichlorophenyl)-8-methyl-2-methylsulfanyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 37, 1.08 g (10.0 mmol) of 2-(aminomethyl)pyridine and 0.5 mL of dimethylformamide was heated with stirring in a 130° C. oil bath. After 2 minutes, solution was complete. After 2 hours, the exc...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Monosulfide
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1.c1ccncc1
Other
CN(C=O)C
130
0.033333
CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1.NCc1ccccn1>CN(C=O)C>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(NCc3ccccn3)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-f149ec04b04c43cd9da4e5fa56e0fec3
CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1.NCc1cccnc1>>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(NCc3cccnc3)nc21
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)SC)N(C1=O)C.NCC=1C=NC=CC1>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NCC=2C=NC=CC2)N(C1=O)C
CS[c:18]1[n:17][cH:16][c:15]2[cH:14][c:5](-[c:6]3[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]3[Cl:13])[c:3](=[O:4])[n:2]([CH3:1])[c:28]2[n:27]1.[NH2:19][CH2:20][c:21]1[cH:22][cH:23][cH:24][n:25][cH:26]1>>[CH3:1][n:2]1[c:3](=[O:4])[c:5](-[c:6]2[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]2[Cl:13])[cH:14][c:15]2[cH:16][n:17][c:18](...
CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1.NCc1cccnc1
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(NCc3cccnc3)nc21
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
df9d6a54bbeb74919f9913aad742e0b7c3ffefcaa8d2bb485e4914ba80c410ee
88e0224d19b2dce8f9987d52554afb32090d36ff7ee19e89dc5bf66d30974ec4
O=c1[nH]c2nc(NCc3cccnc3)ncc2cc1-c1ccccc1
C-S-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[#7;a:10]:[c:11]:[c:12]-[C:13]-[NH2;D1;+0:14]>>[#7;a:10]:[c:11]:[c:12]-[C:13]-[NH;D2;+0:14]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9]
null
[]
null
null
null
null
This compound was prepared by a procedure similar to that described in Example 49 starting with 0.165 g (0.47 mmol) of 6-(2,6-dichlorophenyl)-8-methyl-2-methylsulfanyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 37 and 1.08 g (10.0 mmol) of 3-(aminomethyl)-pyridine yielding 0.053 g of pure product; mp 224°-226° C. Condi...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Monosulfide
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1.c1ccncc1
Other
null
null
null
CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1.NCc1cccnc1>>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(NCc3cccnc3)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-3a132906f38a4c07b3d4eb7a38743313
CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1.NCCc1ccccn1>>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(NCCc3ccccn3)nc21
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)SC)N(C1=O)C.NCCC1=NC=CC=C1>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NCCC2=NC=CC=C2)N(C1=O)C
CS[c:18]1[n:17][cH:16][c:15]2[cH:14][c:5](-[c:6]3[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]3[Cl:13])[c:3](=[O:4])[n:2]([CH3:1])[c:29]2[n:28]1.[NH2:19][CH2:20][CH2:21][c:22]1[cH:23][cH:24][cH:25][cH:26][n:27]1>>[CH3:1][n:2]1[c:3](=[O:4])[c:5](-[c:6]2[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]2[Cl:13])[cH:14][c:15]2[cH:16][n:17...
CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1.NCCc1ccccn1
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(NCCc3ccccn3)nc21
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
df9d6a54bbeb74919f9913aad742e0b7c3ffefcaa8d2bb485e4914ba80c410ee
88e0224d19b2dce8f9987d52554afb32090d36ff7ee19e89dc5bf66d30974ec4
O=c1[nH]c2nc(NCCc3ccccn3)ncc2cc1-c1ccccc1
C-S-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[C:10]-[C:11]-[NH2;D1;+0:12]>>[C:10]-[C:11]-[NH;D2;+0:12]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9]
null
[]
null
null
null
null
This compound was prepared by a procedure similar to that described in Example 49 starting with 0.165 g (0.47 mmol) of 6-(2,6-dichlorophenyl)-8-methyl-2-methylsulfanyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 37 and 1.00 g (8.20 mmol) of 2-(2-aminoethyl)-pyridine yielding 0.082 g of pure product; mp 173°-174° C. Cond...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Monosulfide
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1.c1ccncc1
Other
null
null
null
CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1.NCCc1ccccn1>>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(NCCc3ccccn3)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-16b1b5b57c634a8aa4a0c762c66831e2
COc1ccccc1N1CCN(CCCN)CC1.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1>>COc1ccccc1N1CCN(CCCNc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)CC1
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)SC)N(C1=O)C.NCCCN1CCN(CC1)C1=C(C=CC=C1)OC>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NCCCN2CCN(CC2)C2=C(C=CC=C2)OC)N(C1=O)C
[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][cH:7][c:8]1[N:9]1[CH2:10][CH2:11][N:12]([CH2:13][CH2:14][CH2:15][NH2:16])[CH2:37][CH2:38]1.CS[c:17]1[n:18][cH:19][c:20]2[cH:21][c:22](-[c:23]3[c:24]([Cl:25])[cH:26][cH:27][cH:28][c:29]3[Cl:30])[c:31](=[O:32])[n:33]([CH3:34])[c:35]2[n:36]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][cH:7][...
COc1ccccc1N1CCN(CCCN)CC1.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
COc1ccccc1N1CCN(CCCNc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)CC1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
df9d6a54bbeb74919f9913aad742e0b7c3ffefcaa8d2bb485e4914ba80c410ee
88e0224d19b2dce8f9987d52554afb32090d36ff7ee19e89dc5bf66d30974ec4
O=c1[nH]c2nc(NCCCN3CCN(c4ccccc4)CC3)ncc2cc1-c1ccccc1
C-S-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[C:10]-[C:11]-[NH2;D1;+0:12]>>[C:10]-[C:11]-[NH;D2;+0:12]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9]
null
[]
null
null
null
null
This compound was prepared by a procedure similar to that described in Example 49 starting with 0.165 g (0.47 mmol) of 6-(2,6-dichlorophenyl)-8-methyl-2-methylsulfanyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 37 and 1.00 g (4.00 mmol) of 1-(3-aminopropyl)-4-(2-methoxyphenyl)piperazine yielding 0.103 g of pure product...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Monosulfide
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.C1C[NH]CC[NH]1.c1cnc2ncncc2c1.c1ccccc1
Other
null
null
null
COc1ccccc1N1CCN(CCCN)CC1.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1>>COc1ccccc1N1CCN(CCCNc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)CC1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-0aaab490559345e3a5659881e04302db
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.Nc1ccccc1>>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3ccccc3)nc21
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)S(=O)(=O)C)N(C1=O)C.NC1=CC=CC=C1>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NC2=CC=CC=C2)N(C1=O)C
CS(=O)(=O)[c:18]1[n:17][cH:16][c:15]2[cH:14][c:5](-[c:6]3[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]3[Cl:13])[c:3](=[O:4])[n:2]([CH3:1])[c:27]2[n:26]1.[NH2:19][c:20]1[cH:21][cH:22][cH:23][cH:24][cH:25]1>>[CH3:1][n:2]1[c:3](=[O:4])[c:5](-[c:6]2[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]2[Cl:13])[cH:14][c:15]2[cH:16][n:17][c:18]...
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.Nc1ccccc1
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3ccccc3)nc21
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1[nH]c2nc(Nc3ccccc3)ncc2cc1-c1ccccc1
C-S(=O)(=O)-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[C;D1;H3:8]-[#7;a:7](:[c:9]):[c:5]1:[#7;a:6]:[c;H0;D3;+0:1](-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13]):[#7;a:2]:[c:3]:[c:4]:1
null
[]
184
CELSIUS
null
null
A solution of 0.113 g (0.29 mmol) of 6-(2,6-dichlorophenyl)-2-methanesulfonyl-8-methyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 39 in 1.00 g (10.70 mmol) of aniline was maintained at reflux (184° C.) for 3 minutes. Most of the excess aniline was evaporated at reduced pressure. The remaining gum was dissolved in 1.0 m...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1.c1ccccc1
HO-
null
184
null
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.Nc1ccccc1>>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3ccccc3)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-2fa6392e84c549aa85701a13e6abad4d
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.Nc1ccc(Cl)cc1>>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3ccc(Cl)cc3)nc21
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)S(=O)(=O)C)N(C1=O)C.ClC1=CC=C(N)C=C1>>ClC1=CC=C(C=C1)NC=1N=CC2=C(N1)N(C(C(=C2)C2=C(C=CC=C2Cl)Cl)=O)C
CS(=O)(=O)[c:18]1[n:17][cH:16][c:15]2[cH:14][c:5](-[c:6]3[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]3[Cl:13])[c:3](=[O:4])[n:2]([CH3:1])[c:28]2[n:27]1.[NH2:19][c:20]1[cH:21][cH:22][c:23]([Cl:24])[cH:25][cH:26]1>>[CH3:1][n:2]1[c:3](=[O:4])[c:5](-[c:6]2[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]2[Cl:13])[cH:14][c:15]2[cH:16][n:1...
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.Nc1ccc(Cl)cc1
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3ccc(Cl)cc3)nc21
null
null
C(C)(=O)OCC
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1[nH]c2nc(Nc3ccccc3)ncc2cc1-c1ccccc1
C-S(=O)(=O)-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[C;D1;H3:8]-[#7;a:7](:[c:9]):[c:5]1:[#7;a:6]:[c;H0;D3;+0:1](-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13]):[#7;a:2]:[c:3]:[c:4]:1
null
[]
238
CELSIUS
5
MINUTE
A mixture of 0.113 g (0.29 mmol) of 6-(2,6-dichlorophenyl)-2-methanesulfonyl-8-methyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 39 in 0.50 g (3.90 mmol) of 4-chloroaniline was heated, with stirring, at the boiling point (238° C.) for 5 minutes. Ethyl acetate (3 mL) was added to the cooled dark blue reaction solution. ...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1.c1ccccc1
HO-
C(C)(=O)OCC
238
0.083333
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.Nc1ccc(Cl)cc1>C(C)(=O)OCC>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3ccc(Cl)cc3)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-229e6ead42474df5b581ec87f76dc9f1
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.Nc1ccc2c(c1)OCO2>>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3ccc4c(c3)OCO4)nc21
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)S(=O)(=O)C)N(C1=O)C.C1OC=2C=C(N)C=CC2O1>>O1COC2=C1C=CC(=C2)NC=2N=CC1=C(N2)N(C(C(=C1)C1=C(C=CC=C1Cl)Cl)=O)C
CS(=O)(=O)[c:18]1[n:17][cH:16][c:15]2[cH:14][c:5](-[c:6]3[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]3[Cl:13])[c:3](=[O:4])[n:2]([CH3:1])[c:30]2[n:29]1.[NH2:19][c:20]1[cH:21][cH:22][c:23]2[c:24]([cH:25]1)[O:26][CH2:27][O:28]2>>[CH3:1][n:2]1[c:3](=[O:4])[c:5](-[c:6]2[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]2[Cl:13])[cH:14][c:1...
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.Nc1ccc2c(c1)OCO2
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3ccc4c(c3)OCO4)nc21
null
null
C(C)(=O)OCC
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1[nH]c2nc(Nc3ccc4c(c3)OCO4)ncc2cc1-c1ccccc1
C-S(=O)(=O)-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[C;D1;H3:8]-[#7;a:7](:[c:9]):[c:5]1:[#7;a:6]:[c;H0;D3;+0:1](-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13]):[#7;a:2]:[c:3]:[c:4]:1
null
[]
200
CELSIUS
null
null
A mixture of 0.113 g (0.29 mmol) of 6-(2,6-dichlorophenyl)-2-methanesulfonyl-8-methyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 39 and 0.50 g (3.70 mmol) of 3,4-methylenedioxyaniline was heated, with stirring, in a 200° C. oil bath. The resulting solution was heated for 5 minutes and cooled to room temperature. Ethyl ...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1.c1ccc2c(c1)OCO2
HO-
C(C)(=O)OCC
200
null
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.Nc1ccc2c(c1)OCO2>C(C)(=O)OCC>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3ccc4c(c3)OCO4)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-93c51878ae8a413eb4db15ce380f4843
CN1CCN(CCCCN)CC1.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1>>CN1CCN(CCCCNc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)CC1
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)SC)N(C1=O)C.NCCCCN1CCN(CC1)C>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NCCCCN2CCN(CC2)C)N(C1=O)C
[CH3:1][N:2]1[CH2:3][CH2:4][N:5]([CH2:6][CH2:7][CH2:8][CH2:9][NH2:10])[CH2:31][CH2:32]1.CS[c:11]1[n:12][cH:13][c:14]2[cH:15][c:16](-[c:17]3[c:18]([Cl:19])[cH:20][cH:21][cH:22][c:23]3[Cl:24])[c:25](=[O:26])[n:27]([CH3:28])[c:29]2[n:30]1>>[CH3:1][N:2]1[CH2:3][CH2:4][N:5]([CH2:6][CH2:7][CH2:8][CH2:9][NH:10][c:11]2[n:12][c...
CN1CCN(CCCCN)CC1.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
CN1CCN(CCCCNc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)CC1
null
null
CCOCC
Heteroatom Alkylation and Arylation
OtherReaction
df9d6a54bbeb74919f9913aad742e0b7c3ffefcaa8d2bb485e4914ba80c410ee
88e0224d19b2dce8f9987d52554afb32090d36ff7ee19e89dc5bf66d30974ec4
O=c1[nH]c2nc(NCCCCN3CCNCC3)ncc2cc1-c1ccccc1
C-S-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[C:10]-[C:11]-[NH2;D1;+0:12]>>[C:10]-[C:11]-[NH;D2;+0:12]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9]
null
[]
170
CELSIUS
2
MINUTE
A mixture of 0.152 g (0.43 mmol) of 6-(2,6-dichlorophenyl)-8-methyl-2-methylsulfanyl-8-pyrido[2,3-d]pyrimidin-7-one of Example 37 and 0.50 g (2.90 mmol) of 1-(4-aminobutyl)-4-methylpiperazine was heated with stirring in a 170° C. oil bath. After 2 minutes, solution was complete. After 2 hours, the solution was cooled t...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Monosulfide
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
C1C[NH]CC[NH]1.c1cnc2ncncc2c1.c1ccccc1
Other
CCOCC
170
0.033333
CN1CCN(CCCCN)CC1.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1>CCOCC>CN1CCN(CCCCNc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)CC1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-3191b5ba687c4a38ba69160188ee969d
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.NC1CCCCC1>>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(NC3CCCCC3)nc21
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)S(=O)(=O)C)N(C1=O)C.C1(CCCCC1)N>>C1(CCCCC1)NC=1N=CC2=C(N1)N(C(C(=C2)C2=C(C=CC=C2Cl)Cl)=O)C
CS(=O)(=O)[c:18]1[n:17][cH:16][c:15]2[cH:14][c:5](-[c:6]3[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]3[Cl:13])[c:3](=[O:4])[n:2]([CH3:1])[c:27]2[n:26]1.[NH2:19][CH:20]1[CH2:21][CH2:22][CH2:23][CH2:24][CH2:25]1>>[CH3:1][n:2]1[c:3](=[O:4])[c:5](-[c:6]2[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]2[Cl:13])[cH:14][c:15]2[cH:16][n:17]...
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.NC1CCCCC1
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(NC3CCCCC3)nc21
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1[nH]c2nc(NC3CCCCC3)ncc2cc1-c1ccccc1
C-S(=O)(=O)-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[C:10]-[C:11](-[NH2;D1;+0:12])-[C:13]>>[C:10]-[C:11](-[NH;D2;+0:12]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9])-[C:13]
null
[]
134
CELSIUS
null
null
A mixture of 0.100 g (0.26 mmol) of 6-(2,6-dichlorophenyl)-2-methanesulfonyl-8-methyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 39 and 0.300 g (3.00 mmol) of cyclohexylamine was heated to the boiling point (134° C.). The resulting solution was heated at reflux for 2 minutes. Most of the excess amine was evaporated at ...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1.C1CCCCC1
HO-
null
134
null
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.NC1CCCCC1>>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(NC3CCCCC3)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-7c0d2f4521364c5dbc8d4b38d2935639
Cc1ccc(N)cc1.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21>>Cc1ccc(NN2C=c3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3=NC2)cc1
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)S(=O)(=O)C)N(C1=O)C.CC1=CC=C(N)C=C1>>ClC1=C(C(=CC=C1)Cl)C1=CC=2C(=NCN(C2)NC2=CC=C(C=C2)C)N(C1=O)C
[CH3:1][c:2]1[cH:3][cH:4][c:5]([NH2:6])[cH:27][cH:28]1.CS(=O)(=O)[c:26]1[n:7][cH:8][c:9]2[cH:10][c:11](-[c:12]3[c:13]([Cl:14])[cH:15][cH:16][cH:17][c:18]3[Cl:19])[c:20](=[O:21])[n:22]([CH3:23])[c:24]2[n:25]1>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([NH:6][N:7]2[CH:8]=[c:9]3[cH:10][c:11](-[c:12]4[c:13]([Cl:14])[cH:15][cH:16][cH:...
Cc1ccc(N)cc1.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21
Cc1ccc(NN2C=c3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3=NC2)cc1
null
null
null
Miscellaneous
OtherReaction
2261235475fc28ea339785b3b09ba6fac4ff17f1ffda032b5b9b36e8c4844217
01029f5a8ad6bf4b4408b4ba553d43977ce413937313c5e69fb72996996c7328
O=c1[nH]c2c(cc1-c1ccccc1)=CN(Nc1ccccc1)CN=2
C-S(=O)(=O)-[c;H0;D3;+0:1]1:[n;H0;D2;+0:2]:[c;H0;D3;+0:3]2:[#7;a:4](-[C;D1;H3:5]):[c:6]:[c:7]:[c:8]:[c;H0;D3;+0:9]:2:[cH;D2;+0:10]:[n;H0;D2;+0:11]:1.[NH2;D1;+0:12]-[c:13](:[c:14]):[c:15]>>[C;D1;H3:5]-[#7;a:4]1:[c:6]:[c:7]:[c:8]:[c;H0;D3;+0:9]2:[c;H0;D3;+0:3]:1=[N;H0;D2;+0:2]-[CH2;D2;+0:1]-[N;H0;D3;+0:11](-[NH;D2;+0:12]...
null
[]
180
CELSIUS
null
null
A mixture of 0.113 g (0.29 mmol) of 6-(2,6-dichlorophenyl)-2-methanesulfonyl-8-methyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 39 and 0.50 g (4.70 mmol) of 4-methylaniline was heated, with stirring, in a 180° C. oil bath. The resulting solution was heated for 10 minutes. Much of the excess 4-methylaniline was evapora...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Hydrazine
c1cnc2ncncc2c1
C1=c2cccnc2=NC[NH]1
c1ccccc1.C1=c2cccnc2=NC[NH]1.c1ccccc1
HO-
null
180
null
Cc1ccc(N)cc1.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21>>Cc1ccc(NN2C=c3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3=NC2)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-2385e0240fd44243a34f8caa93efa84f
COc1ccc(N)cc1.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21>>COc1ccc(Nc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)cc1
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)S(=O)(=O)C)N(C1=O)C.COC1=CC=C(N)C=C1>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NC2=CC=C(C=C2)OC)N(C1=O)C
[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([NH2:7])[cH:28][cH:29]1.CS(=O)(=O)[c:8]1[n:9][cH:10][c:11]2[cH:12][c:13](-[c:14]3[c:15]([Cl:16])[cH:17][cH:18][cH:19][c:20]3[Cl:21])[c:22](=[O:23])[n:24]([CH3:25])[c:26]2[n:27]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([NH:7][c:8]2[n:9][cH:10][c:11]3[cH:12][c:13](-[c:14]4[c:15]([Cl:16])[...
COc1ccc(N)cc1.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21
COc1ccc(Nc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)cc1
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1[nH]c2nc(Nc3ccccc3)ncc2cc1-c1ccccc1
C-S(=O)(=O)-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](:[c:4]:[c:5]:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[C;D1;H3:8]-[#7;a:7](:[c:9]):[c:3]1:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13]):[#7;a:6]:[c:5]:[c:4]:1
null
[]
180
CELSIUS
null
null
A mixture of 0.113 g (0.29 mmol) of 6-(2,6-dichlorophenyl)-2-methanesulfonyl-8-methyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 39 and 0.50 g (4.10 mmol) of 4-methoxyaniline was heated, with stirring, in a 180° C. oil bath. The resulting solution was heated for 10 minutes. Much of the excess aniline was evaporated at ...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1.c1ccccc1
HO-
null
180
null
COc1ccc(N)cc1.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21>>COc1ccc(Nc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-8675cbe68b9f48d288dee7a6e5c59cad
CC(=O)OC(C)=O.CCn1c(=N)c(-c2c(Cl)cccc2Cl)cc2cnc(SC)nc21>>CCn1c(=NC(C)=O)c(-c2c(Cl)cccc2Cl)cc2cnc(SC)nc21
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)SC)N(C1=N)CC.C(C)(=O)OC(C)=O>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)SC)N(C1=NC(C)=O)CC
CC(=O)O[C:6]([CH3:7])=[O:8].[CH3:1][CH2:2][n:3]1[c:4](=[NH:5])[c:9](-[c:10]2[c:11]([Cl:12])[cH:13][cH:14][cH:15][c:16]2[Cl:17])[cH:18][c:19]2[cH:20][n:21][c:22]([S:23][CH3:24])[n:25][c:26]12>>[CH3:1][CH2:2][n:3]1[c:4](=[N:5][C:6]([CH3:7])=[O:8])[c:9](-[c:10]2[c:11]([Cl:12])[cH:13][cH:14][cH:15][c:16]2[Cl:17])[cH:18][c:...
CC(=O)OC(C)=O.CCn1c(=N)c(-c2c(Cl)cccc2Cl)cc2cnc(SC)nc21
CCn1c(=NC(C)=O)c(-c2c(Cl)cccc2Cl)cc2cnc(SC)nc21
null
null
null
Acylation
Aminolysis of esters
868ba94f028b30e9347f1568001d166d126ab48ad34862bd252bb72f87967edd
93289da630dbaf2d9339c4212dcd342dfbcc29df4e79a63418a0fd9f589abdc1
N=c1[nH]c2ncncc2cc1-c1ccccc1
C-C(=O)-O-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[#7;a:4]:[c:5]:[#7;a:6](-[C:7]):[c:8](=[NH;D1;+0:9]):[c:10]>>[#7;a:4]:[c:5]:[#7;a:6](-[C:7]):[c:8](=[N;H0;D2;+0:9]-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3]):[c:10]
null
[]
null
null
null
null
A mixture of 2.70 g (7.40 mmol) of 6-(2,6-dichlorophenyl)-8-ethyl-2-methylsulfanyl-8H-pyrido[2,3-d]pyrimidin-7-ylideneamine of Example 65 and 15 mL of acetic anhydride was heated with stirring to the boiling point. The resulting solution was heated at reflux for 5 minutes and concentrated at reduced pressure to ca. 8 m...
10.6084/m9.figshare.5104873.v1
null
Anhydride
null
null
null
c1ccccc1.c1cnc2ncncc2c1
HO-
null
null
null
CC(=O)OC(C)=O.CCn1c(=N)c(-c2c(Cl)cccc2Cl)cc2cnc(SC)nc21>>CCn1c(=NC(C)=O)c(-c2c(Cl)cccc2Cl)cc2cnc(SC)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-4ca4e30594e44f88b0f99fc7322a410a
CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.Nc1ccccc1>>CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3ccccc3)nc21
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)S(=O)(=O)C)N(C1=O)CC.NC1=CC=CC=C1>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NC2=CC=CC=C2)N(C1=O)CC
CS(=O)(=O)[c:19]1[n:18][cH:17][c:16]2[cH:15][c:6](-[c:7]3[c:8]([Cl:9])[cH:10][cH:11][cH:12][c:13]3[Cl:14])[c:4](=[O:5])[n:3]([CH2:2][CH3:1])[c:28]2[n:27]1.[NH2:20][c:21]1[cH:22][cH:23][cH:24][cH:25][cH:26]1>>[CH3:1][CH2:2][n:3]1[c:4](=[O:5])[c:6](-[c:7]2[c:8]([Cl:9])[cH:10][cH:11][cH:12][c:13]2[Cl:14])[cH:15][c:16]2[cH...
CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.Nc1ccccc1
CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3ccccc3)nc21
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1[nH]c2nc(Nc3ccccc3)ncc2cc1-c1ccccc1
C-S(=O)(=O)-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C:8]):[c:9].[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[C:8]-[#7;a:7](:[c:9]):[c:5]1:[#7;a:6]:[c;H0;D3;+0:1](-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13]):[#7;a:2]:[c:3]:[c:4]:1
null
[]
195
CELSIUS
null
null
A mixture of 0.134 g (0.33 mmol) of 6-(2,6-dichlorophenyl)-8-ethyl-2-methanesulfonyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 68 and 0.500 g (5.40 mmol) of aniline was heated with stirring in a 195° C. oil bath to reflux. The resulting solution was maintained at reflux for 5 minutes. Most of the excess aniline was ev...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1.c1ccccc1
HO-
null
195
null
CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.Nc1ccccc1>>CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3ccccc3)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-2a5b023190f34924a6abcd11c41e178a
COc1ccccc1N.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21>>COc1ccccc1Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)S(=O)(=O)C)N(C1=O)C.COC1=C(N)C=CC=C1>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NC2=C(C=CC=C2)OC)N(C1=O)C
[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][cH:7][c:8]1[NH2:9].CS(=O)(=O)[c:10]1[n:11][cH:12][c:13]2[cH:14][c:15](-[c:16]3[c:17]([Cl:18])[cH:19][cH:20][cH:21][c:22]3[Cl:23])[c:24](=[O:25])[n:26]([CH3:27])[c:28]2[n:29]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][cH:7][c:8]1[NH:9][c:10]1[n:11][cH:12][c:13]2[cH:14][c:15](-[c:16]3[c:1...
COc1ccccc1N.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21
COc1ccccc1Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
null
null
CCOCC
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1[nH]c2nc(Nc3ccccc3)ncc2cc1-c1ccccc1
C-S(=O)(=O)-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[C;D1;H3:8]-[#7;a:7](:[c:9]):[c:5]1:[#7;a:6]:[c;H0;D3;+0:1](-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13]):[#7;a:2]:[c:3]:[c:4]:1
null
[]
175
CELSIUS
null
null
A mixture of 0.113 g (0.29 mmol) of 6-(2,6-dichlorophenyl)-2-methanesulfonyl-8-methyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 39 and 0.50 g (4.10 mmol) of 2-methoxyaniline was heated, with stirring, in a 175° C. oil bath. The resulting solution was heated for 5 minutes and cooled to room temperature. Ether (2 mL) wa...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1.c1ccccc1
HO-
CCOCC
175
null
COc1ccccc1N.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21>CCOCC>COc1ccccc1Nc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-eda16d28ddde4d29b868c0f9438c5f73
COc1ccc(N)cc1C.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21>>COc1ccc(Nc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)cc1C
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)S(=O)(=O)C)N(C1=O)C.CC=1C=C(N)C=CC1OC>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NC2=CC(=C(C=C2)OC)C)N(C1=O)C
[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([NH2:7])[cH:28][c:29]1[CH3:30].CS(=O)(=O)[c:8]1[n:9][cH:10][c:11]2[cH:12][c:13](-[c:14]3[c:15]([Cl:16])[cH:17][cH:18][cH:19][c:20]3[Cl:21])[c:22](=[O:23])[n:24]([CH3:25])[c:26]2[n:27]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([NH:7][c:8]2[n:9][cH:10][c:11]3[cH:12][c:13](-[c:14]4[c:15]([C...
COc1ccc(N)cc1C.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21
COc1ccc(Nc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)cc1C
null
null
CCOCC
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1[nH]c2nc(Nc3ccccc3)ncc2cc1-c1ccccc1
C-S(=O)(=O)-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](:[c:4]:[c:5]:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[C;D1;H3:8]-[#7;a:7](:[c:9]):[c:3]1:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13]):[#7;a:6]:[c:5]:[c:4]:1
null
[]
165
CELSIUS
null
null
A mixture of 0.113 g (0.29 mmol) of 6-(2,6-dichlorophenyl)-2-methanesulfonyl-8-methyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 39 and 0.40 g (2.90 mmol) of 3-methyl-4-methoxyaniline was heated, with stirring, in a 165° C. oil bath. The resulting solution was heated for 5 minutes and cooled to room temperature. Ether ...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1.c1ccccc1
HO-
CCOCC
165
null
COc1ccc(N)cc1C.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21>CCOCC>COc1ccc(Nc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)cc1C
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-68d8ae5623a045faa4752c54188d8074
CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.COc1ccc(N)cc1>>CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3ccc(OC)cc3)nc21
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)S(=O)(=O)C)N(C1=O)CC.COC1=CC=C(N)C=C1>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NC2=CC=C(C=C2)OC)N(C1=O)CC
CS(=O)(=O)[c:19]1[n:18][cH:17][c:16]2[cH:15][c:6](-[c:7]3[c:8]([Cl:9])[cH:10][cH:11][cH:12][c:13]3[Cl:14])[c:4](=[O:5])[n:3]([CH2:2][CH3:1])[c:30]2[n:29]1.[NH2:20][c:21]1[cH:22][cH:23][c:24]([O:25][CH3:26])[cH:27][cH:28]1>>[CH3:1][CH2:2][n:3]1[c:4](=[O:5])[c:6](-[c:7]2[c:8]([Cl:9])[cH:10][cH:11][cH:12][c:13]2[Cl:14])[c...
CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.COc1ccc(N)cc1
CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3ccc(OC)cc3)nc21
null
O
CN(C=O)C
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1[nH]c2nc(Nc3ccccc3)ncc2cc1-c1ccccc1
C-S(=O)(=O)-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C:8]):[c:9].[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[C:8]-[#7;a:7](:[c:9]):[c:5]1:[#7;a:6]:[c;H0;D3;+0:1](-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13]):[#7;a:2]:[c:3]:[c:4]:1
null
[]
null
null
null
null
A solution of 0.100 g (0.25 mmol) of 6-(2,6-dichlorophenyl)-8-ethyl-2-methanesulfonyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 68 and 0.061 g (0.50 mmol) of 4-methoxyaniline in 0.5 mL of dimethylformamide was heated at reflux for 10 minutes. Three drops of water were added. Crystals separated on inducement. An additi...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1.c1ccccc1
HO-
O.CN(C=O)C
null
null
CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.COc1ccc(N)cc1>O.CN(C=O)C>CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3ccc(OC)cc3)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-e03019db057645d990f6974409cc35bc
CCOc1ccc(N)cc1.CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21>>CCOc1ccc(Nc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(CC)c3n2)cc1
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)S(=O)(=O)C)N(C1=O)CC.C(C)OC1=CC=C(N)C=C1>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NC2=CC=C(C=C2)OCC)N(C1=O)CC
[CH3:1][CH2:2][O:3][c:4]1[cH:5][cH:6][c:7]([NH2:8])[cH:30][cH:31]1.CS(=O)(=O)[c:9]1[n:10][cH:11][c:12]2[cH:13][c:14](-[c:15]3[c:16]([Cl:17])[cH:18][cH:19][cH:20][c:21]3[Cl:22])[c:23](=[O:24])[n:25]([CH2:26][CH3:27])[c:28]2[n:29]1>>[CH3:1][CH2:2][O:3][c:4]1[cH:5][cH:6][c:7]([NH:8][c:9]2[n:10][cH:11][c:12]3[cH:13][c:14](...
CCOc1ccc(N)cc1.CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21
CCOc1ccc(Nc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(CC)c3n2)cc1
null
null
C(C)(=O)O.O
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1[nH]c2nc(Nc3ccccc3)ncc2cc1-c1ccccc1
C-S(=O)(=O)-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C:8]):[c:9].[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[C:8]-[#7;a:7](:[c:9]):[c:5]1:[#7;a:6]:[c;H0;D3;+0:1](-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13]):[#7;a:2]:[c:3]:[c:4]:1
null
[]
null
null
null
null
A mixture of 0.150 g (0.38 mmol) of 6-(2,6-dichlorophenyl)-8-ethyl-2-methanesulfonyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 68 and 0.500 g (3.60 mmol) of 4-ethoxyaniline was fused in a 160° C. oil bath for 10 minutes. The dark violet melt was cooled and dissolved in 1 mL of warm glacial acetic acid. This solution w...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1.c1ccccc1
HO-
C(C)(=O)O.O
null
null
CCOc1ccc(N)cc1.CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21>C(C)(=O)O.O>CCOc1ccc(Nc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(CC)c3n2)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-81f4c40125694e76a49bac3d81b5f484
CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.COc1ccc(N)cc1OC>>CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3ccc(OC)c(OC)c3)nc21
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)S(=O)(=O)C)N(C1=O)CC.COC=1C=C(N)C=CC1OC>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NC2=CC(=C(C=C2)OC)OC)N(C1=O)CC
CS(=O)(=O)[c:19]1[n:18][cH:17][c:16]2[cH:15][c:6](-[c:7]3[c:8]([Cl:9])[cH:10][cH:11][cH:12][c:13]3[Cl:14])[c:4](=[O:5])[n:3]([CH2:2][CH3:1])[c:32]2[n:31]1.[NH2:20][c:21]1[cH:22][cH:23][c:24]([O:25][CH3:26])[c:27]([O:28][CH3:29])[cH:30]1>>[CH3:1][CH2:2][n:3]1[c:4](=[O:5])[c:6](-[c:7]2[c:8]([Cl:9])[cH:10][cH:11][cH:12][c...
CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.COc1ccc(N)cc1OC
CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3ccc(OC)c(OC)c3)nc21
null
null
C(C)(=O)O.O
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1[nH]c2nc(Nc3ccccc3)ncc2cc1-c1ccccc1
C-S(=O)(=O)-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C:8]):[c:9].[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[C:8]-[#7;a:7](:[c:9]):[c:5]1:[#7;a:6]:[c;H0;D3;+0:1](-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13]):[#7;a:2]:[c:3]:[c:4]:1
null
[]
160
CELSIUS
null
null
A mixture of 0.150 g (0.38 mmol) of 6-(2,6-dichlorophenyl)-8-ethyl-2-methanesulfonyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 68 and 0.500 g (3.30 mmol) of 3,4-dimethoxyaniline was heated in a 160° C. oil bath for 5 minutes. The dark blue solution was cooled and dissolved in 2 mL of warm glacial acetic acid. This sol...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1.c1ccccc1
HO-
C(C)(=O)O.O
160
null
CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.COc1ccc(N)cc1OC>C(C)(=O)O.O>CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3ccc(OC)c(OC)c3)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-76f6a432b29140da8181c2f2c78550f6
CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.COc1cc(N)cc(OC)c1OC>>CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3cc(OC)c(OC)c(OC)c3)nc21
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)S(=O)(=O)C)N(C1=O)CC.COC=1C=C(N)C=C(C1OC)OC>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NC2=CC(=C(C(=C2)OC)OC)OC)N(C1=O)CC
CS(=O)(=O)[c:19]1[n:18][cH:17][c:16]2[cH:15][c:6](-[c:7]3[c:8]([Cl:9])[cH:10][cH:11][cH:12][c:13]3[Cl:14])[c:4](=[O:5])[n:3]([CH2:2][CH3:1])[c:34]2[n:33]1.[NH2:20][c:21]1[cH:22][c:23]([O:24][CH3:25])[c:26]([O:27][CH3:28])[c:29]([O:30][CH3:31])[cH:32]1>>[CH3:1][CH2:2][n:3]1[c:4](=[O:5])[c:6](-[c:7]2[c:8]([Cl:9])[cH:10][...
CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.COc1cc(N)cc(OC)c1OC
CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3cc(OC)c(OC)c(OC)c3)nc21
null
null
C(C)(=O)O.O
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1[nH]c2nc(Nc3ccccc3)ncc2cc1-c1ccccc1
C-S(=O)(=O)-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C:8]):[c:9].[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[C:8]-[#7;a:7](:[c:9]):[c:5]1:[#7;a:6]:[c;H0;D3;+0:1](-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13]):[#7;a:2]:[c:3]:[c:4]:1
null
[]
160
CELSIUS
null
null
A mixture of 0.150 g (0.38 mmol) of 6-(2,6-dichlorophenyl)-8-ethyl-2-methanesulfonyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 68 and 0.500 g (2.70 mmol) of 3,4,5-trimethoxyaniline was heated in a 160° C. oil bath for 5 minutes. The dark solution was cooled and dissolved in 2 mL of warm glacial acetic acid. This solut...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1.c1ccccc1
HO-
C(C)(=O)O.O
160
null
CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.COc1cc(N)cc(OC)c1OC>C(C)(=O)O.O>CCn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3cc(OC)c(OC)c(OC)c3)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-e995bd2a805644e4b3e1fc791d696150
CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1.Nc1cccnc1>>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3cccnc3)nc21
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)SC)N(C1=O)C.NC=1C=NC=CC1.Cl.NC=1C=NC=CC1>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NC=2C=NC=CC2)N(C1=O)C
CS[c:18]1[n:17][cH:16][c:15]2[cH:14][c:5](-[c:6]3[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]3[Cl:13])[c:3](=[O:4])[n:2]([CH3:1])[c:27]2[n:26]1.[NH2:19][c:20]1[cH:21][cH:22][cH:23][n:24][cH:25]1>>[CH3:1][n:2]1[c:3](=[O:4])[c:5](-[c:6]2[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]2[Cl:13])[cH:14][c:15]2[cH:16][n:17][c:18]([NH:19][...
CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1.Nc1cccnc1
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3cccnc3)nc21
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
df9d6a54bbeb74919f9913aad742e0b7c3ffefcaa8d2bb485e4914ba80c410ee
88e0224d19b2dce8f9987d52554afb32090d36ff7ee19e89dc5bf66d30974ec4
O=c1[nH]c2nc(Nc3cccnc3)ncc2cc1-c1ccccc1
C-S-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]:[#7;a:14]:[c:15]>>[C;D1;H3:8]-[#7;a:7](:[c:9]):[c:5]1:[#7;a:6]:[c;H0;D3;+0:1](-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13]:[#7;a:14]:[c:15]):[#7;a:2]:[c:3]:[c:4]:1
null
[]
210
CELSIUS
1
HOUR
A mixture of 0.165 g (0.47 mmol) of 6-(2,6-dichlorophenyl)-8-methyl-2-methylsulfanyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 37, 0.500 g (5.30 mmol) of 3-aminopyridine base, and 0.066 g (0.50 mmol) of 3-aminopyridine hydrochloride was heated with stirring in a 210° C. oil bath for 1 hour. Water (5 mL) was added to t...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Monosulfide
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1.c1ccncc1
Other
O
210
1
CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1.Nc1cccnc1>O>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3cccnc3)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-0ccd6005f4ca42f39fa580909f4210c7
CCN(CC)CCOc1ccc(N)cc1.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1>>CCN(CC)CCOc1ccc(Nc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)cc1
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)SC)N(C1=O)C.C(C)N(CCOC1=CC=C(N)C=C1)CC.COCCOCCOC>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NC2=CC=C(C=C2)OCCN(CC)CC)N(C1=O)C
[CH3:1][CH2:2][N:3]([CH2:4][CH3:5])[CH2:6][CH2:7][O:8][c:9]1[cH:10][cH:11][c:12]([NH2:13])[cH:34][cH:35]1.CS[c:14]1[n:15][cH:16][c:17]2[cH:18][c:19](-[c:20]3[c:21]([Cl:22])[cH:23][cH:24][cH:25][c:26]3[Cl:27])[c:28](=[O:29])[n:30]([CH3:31])[c:32]2[n:33]1>>[CH3:1][CH2:2][N:3]([CH2:4][CH3:5])[CH2:6][CH2:7][O:8][c:9]1[cH:1...
CCN(CC)CCOc1ccc(N)cc1.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
CCN(CC)CCOc1ccc(Nc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)cc1
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
df9d6a54bbeb74919f9913aad742e0b7c3ffefcaa8d2bb485e4914ba80c410ee
88e0224d19b2dce8f9987d52554afb32090d36ff7ee19e89dc5bf66d30974ec4
O=c1[nH]c2nc(Nc3ccccc3)ncc2cc1-c1ccccc1
C-S-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[C;D1;H3:8]-[#7;a:7](:[c:9]):[c:5]1:[#7;a:6]:[c;H0;D3;+0:1](-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13]):[#7;a:2]:[c:3]:[c:4]:1
null
[]
150
CELSIUS
null
null
A mixture of 0.155 g (0.40 mmol) of 6-(2,6-dichlorophenyl)-8-methyl-2-methylsulfanyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 37, 0.167 g (0.80 mmol) of 4-(2-diethylaminoethoxy)aniline and 1 mL of (2-methoxyethyl)ether (bp 162° C.) was heated with stirring in a 150° C. oil bath. All solid gradually dissolved over a p...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Monosulfide
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1.c1ccccc1
Other
O
150
null
CCN(CC)CCOc1ccc(N)cc1.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1>O>CCN(CC)CCOc1ccc(Nc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-792d4796913a47ddb4ef1bb450d8932d
CN1CCN(CCCCCN)CC1.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1>>CN1CCN(CCCCCNc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)CC1
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)SC)N(C1=O)C.NCCCCCN1CCN(CC1)C>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NCCCCCN2CCN(CC2)C)N(C1=O)C
[CH3:1][N:2]1[CH2:3][CH2:4][N:5]([CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][NH2:11])[CH2:32][CH2:33]1.CS[c:12]1[n:13][cH:14][c:15]2[cH:16][c:17](-[c:18]3[c:19]([Cl:20])[cH:21][cH:22][cH:23][c:24]3[Cl:25])[c:26](=[O:27])[n:28]([CH3:29])[c:30]2[n:31]1>>[CH3:1][N:2]1[CH2:3][CH2:4][N:5]([CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][NH:11...
CN1CCN(CCCCCN)CC1.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1
CN1CCN(CCCCCNc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)CC1
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
df9d6a54bbeb74919f9913aad742e0b7c3ffefcaa8d2bb485e4914ba80c410ee
88e0224d19b2dce8f9987d52554afb32090d36ff7ee19e89dc5bf66d30974ec4
O=c1[nH]c2nc(NCCCCCN3CCNCC3)ncc2cc1-c1ccccc1
C-S-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[C:10]-[C:11]-[NH2;D1;+0:12]>>[C:10]-[C:11]-[NH;D2;+0:12]-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9]
null
[]
null
null
2
MINUTE
A mixture of 0.165 g (0.47 mmol) of 6-(2,6-dichlorophenyl)-8-methyl-2-methylsulfanyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 37 and 0.50 g (2.70 mmol) of 1-(5-aminopentyl)-4-methylpiperazine was heated with stirring in a 180° C. to 185° C. oil bath. After 2 minutes, solution was complete. After 0.5 hour, the solutio...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Monosulfide
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
C1C[NH]CC[NH]1.c1cnc2ncncc2c1.c1ccccc1
Other
O
null
0.033333
CN1CCN(CCCCCN)CC1.CSc1ncc2cc(-c3c(Cl)cccc3Cl)c(=O)n(C)c2n1>O>CN1CCN(CCCCCNc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)CC1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-4b3709d670944052a53ca165365f8b96
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.Nc1cccc(CO)c1>>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3cccc(CO)c3)nc21
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)S(=O)(=O)C)N(C1=O)C.OCC=1C=C(N)C=CC1.C(C)(=O)O>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NC2=CC(=CC=C2)CO)N(C1=O)C
CS(=O)(=O)[c:18]1[n:17][cH:16][c:15]2[cH:14][c:5](-[c:6]3[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]3[Cl:13])[c:3](=[O:4])[n:2]([CH3:1])[c:29]2[n:28]1.[NH2:19][c:20]1[cH:21][cH:22][cH:23][c:24]([CH2:25][OH:26])[cH:27]1>>[CH3:1][n:2]1[c:3](=[O:4])[c:5](-[c:6]2[c:7]([Cl:8])[cH:9][cH:10][cH:11][c:12]2[Cl:13])[cH:14][c:15]2[cH...
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.Nc1cccc(CO)c1
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3cccc(CO)c3)nc21
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1[nH]c2nc(Nc3ccccc3)ncc2cc1-c1ccccc1
C-S(=O)(=O)-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[C;D1;H3:8]-[#7;a:7](:[c:9]):[c:5]1:[#7;a:6]:[c;H0;D3;+0:1](-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13]):[#7;a:2]:[c:3]:[c:4]:1
null
[]
180
CELSIUS
null
null
A mixture of 0.155 g (0.40 mmol) of 6-(2,6-dichlorophenyl)-2-methanesulfonyl-8-methyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 39 and 0.500 g (4.10 mmol) of 3-(hydroxymethyl)aniline was heated in a 180° C. oil bath for 10 minutes. At ca. 120° C., 2 mL of glacial acetic acid were added to dissolve the gum. Water (20 m...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1.c1ccccc1
HO-
O
180
null
Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21.Nc1cccc(CO)c1>O>Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(Nc3cccc(CO)c3)nc21
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-8f36c1ceeca8456d85e3fbff6f422fe7
COc1cc(N)cc(OC)c1.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21>>COc1cc(Nc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)cc(OC)c1
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)S(=O)(=O)C)N(C1=O)C.COC=1C=C(N)C=C(C1)OC.C(C)(=O)O>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NC2=CC(=CC(=C2)OC)OC)N(C1=O)C
[CH3:1][O:2][c:3]1[cH:4][c:5]([NH2:6])[cH:27][c:28]([O:29][CH3:30])[cH:31]1.CS(=O)(=O)[c:7]1[n:8][cH:9][c:10]2[cH:11][c:12](-[c:13]3[c:14]([Cl:15])[cH:16][cH:17][cH:18][c:19]3[Cl:20])[c:21](=[O:22])[n:23]([CH3:24])[c:25]2[n:26]1>>[CH3:1][O:2][c:3]1[cH:4][c:5]([NH:6][c:7]2[n:8][cH:9][c:10]3[cH:11][c:12](-[c:13]4[c:14]([...
COc1cc(N)cc(OC)c1.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21
COc1cc(Nc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)cc(OC)c1
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1[nH]c2nc(Nc3ccccc3)ncc2cc1-c1ccccc1
C-S(=O)(=O)-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](:[c:4]:[c:5]:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[C;D1;H3:8]-[#7;a:7](:[c:9]):[c:3]1:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13]):[#7;a:6]:[c:5]:[c:4]:1
null
[]
160
CELSIUS
null
null
A mixture of 0.155 g (0.40 mmol) of 6-(2,6-dichlorophenyl)-2-methanesulfonyl-8-methyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 39 and 0.400 g (2.60 mmol) of 3,5-dimethoxyaniline was heated in a 160° C. oil bath for 5 minutes. At ca. 100° C., 1 mL of glacial acetic acid was added to the melt to dissolve. Water (10 mL)...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1.c1ccccc1
HO-
O
160
null
COc1cc(N)cc(OC)c1.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21>O>COc1cc(Nc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)cc(OC)c1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-4568d01a95fc402ebb6310c7c420554f
COC(=O)Cc1ccc(N)cc1.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21>>COC(=O)Cc1ccc(Nc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)cc1
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)S(=O)(=O)C)N(C1=O)C.NC1=CC=C(C=C1)CC(=O)OC.C(C)(=O)O>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NC2=CC=C(C=C2)CC(=O)OC)N(C1=O)C
[CH3:1][O:2][C:3](=[O:4])[CH2:5][c:6]1[cH:7][cH:8][c:9]([NH2:10])[cH:31][cH:32]1.CS(=O)(=O)[c:11]1[n:12][cH:13][c:14]2[cH:15][c:16](-[c:17]3[c:18]([Cl:19])[cH:20][cH:21][cH:22][c:23]3[Cl:24])[c:25](=[O:26])[n:27]([CH3:28])[c:29]2[n:30]1>>[CH3:1][O:2][C:3](=[O:4])[CH2:5][c:6]1[cH:7][cH:8][c:9]([NH:10][c:11]2[n:12][cH:13...
COC(=O)Cc1ccc(N)cc1.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21
COC(=O)Cc1ccc(Nc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)cc1
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1[nH]c2nc(Nc3ccccc3)ncc2cc1-c1ccccc1
C-S(=O)(=O)-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3]:[c:4]:[c:5](:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]>>[C;D1;H3:8]-[#7;a:7](:[c:9]):[c:5]1:[#7;a:6]:[c;H0;D3;+0:1](-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13]):[#7;a:2]:[c:3]:[c:4]:1
null
[]
null
null
null
null
A mixture of 0.226 g (0.58 mmol) of 6-(2,6-dichlorophenyl)-2-methanesulfonyl-8-methyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 39 and 0.40 g (2.80 mmol) of 4-aminophenylacetic acid, methyl ester base was heated in a 160° C. to 165° C. oil bath. The resulting solution was heated for 10 minutes and cooled to room tempe...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccccc1.c1cnc2ncncc2c1.c1ccccc1
HO-
O
null
null
COC(=O)Cc1ccc(N)cc1.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21>O>COC(=O)Cc1ccc(Nc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)cc1
ord_dataset-018fd0e1351f4fd09b20fcddd97b4c7a
ord-09f50aa656964facbcc08ceb73b76632
COc1ccc(N)cn1.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21>>COc1ccc(Nc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)cn1
ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)S(=O)(=O)C)N(C1=O)C.NC=1C=CC(=NC1)OC>>ClC1=C(C(=CC=C1)Cl)C1=CC2=C(N=C(N=C2)NC=2C=NC(=CC2)OC)N(C1=O)C
[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([NH2:7])[cH:28][n:29]1.CS(=O)(=O)[c:8]1[n:9][cH:10][c:11]2[cH:12][c:13](-[c:14]3[c:15]([Cl:16])[cH:17][cH:18][cH:19][c:20]3[Cl:21])[c:22](=[O:23])[n:24]([CH3:25])[c:26]2[n:27]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([NH:7][c:8]2[n:9][cH:10][c:11]3[cH:12][c:13](-[c:14]4[c:15]([Cl:16])[c...
COc1ccc(N)cn1.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21
COc1ccc(Nc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)cn1
null
null
O
Heteroatom Alkylation and Arylation
OtherReaction
4829c7fa353840c036de48b4c116a7d68d2d5d8395d0f64d6e8c63d9a9bd4025
f263fb011eaf2f85af25e2af9b0908fb2797226f3495a5d6be9230bf229d4fae
O=c1[nH]c2nc(Nc3cccnc3)ncc2cc1-c1ccccc1
C-S(=O)(=O)-[c;H0;D3;+0:1]1:[#7;a:2]:[c:3](:[c:4]:[c:5]:[#7;a:6]:1):[#7;a:7](-[C;D1;H3:8]):[c:9].[NH2;D1;+0:10]-[c:11](:[c:12]):[c:13]:[#7;a:14]:[c:15]>>[C;D1;H3:8]-[#7;a:7](:[c:9]):[c:3]1:[#7;a:2]:[c;H0;D3;+0:1](-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13]:[#7;a:14]:[c:15]):[#7;a:6]:[c:5]:[c:4]:1
null
[]
160
CELSIUS
null
null
A mixture of 0.155 g (0.40 mmol) of 6-(2,6-dichlorophenyl)-2-methanesulfonyl-8-methyl-8H-pyrido[2,3-d]pyrimidin-7-one of Example 39 and 0.50 g (4.00 mmol) of 5-amino-2-methoxypyridine was heated, with stirring, in a 160° C. oil bath. The resulting solution was heated for 10 minutes and cooled to room temperature. Water...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfone
Secondary amine
c1cnc2ncncc2c1
c1cnc2ncncc2c1
c1ccncc1.c1cnc2ncncc2c1.c1ccccc1
HO-
O
160
null
COc1ccc(N)cn1.Cn1c(=O)c(-c2c(Cl)cccc2Cl)cc2cnc(S(C)(=O)=O)nc21>O>COc1ccc(Nc2ncc3cc(-c4c(Cl)cccc4Cl)c(=O)n(C)c3n2)cn1