dataset_id
large_stringclasses
414 values
reaction_id
large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
reactant_smiles
large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-27da8e1d973d4c9ba83f51d41249d0ee
CC(=O)N=c1sc(C)cn1-c1cccc(C(F)(F)F)c1>>Cc1cn(-c2cccc(C(F)(F)F)c2)c(=N)s1
C(C)(=O)N=C1SC(=CN1C1=CC(=CC=C1)C(F)(F)F)C.Cl>>N=C1SC(=CN1C1=CC(=CC=C1)C(F)(F)F)C
CC(=O)[N:16]=[c:15]1[n:4](-[c:5]2[cH:6][cH:7][cH:8][c:9]([C:10]([F:11])([F:12])[F:13])[cH:14]2)[cH:3][c:2]([CH3:1])[s:17]1>>[CH3:1][c:2]1[cH:3][n:4](-[c:5]2[cH:6][cH:7][cH:8][c:9]([C:10]([F:11])([F:12])[F:13])[cH:14]2)[c:15](=[NH:16])[s:17]1
CC(=O)N=c1sc(C)cn1-c1cccc(C(F)(F)F)c1
Cc1cn(-c2cccc(C(F)(F)F)c2)c(=N)s1
null
null
C(C)O.O
Reduction
OtherReaction
0bc3968b35f0839c230afb4215314da278abd4e1f10e42ec3012c5512de49ea5
312e9350dcad67590617294c0eb017edf0b9fbfe6133c06a3f393b871a889092
N=c1sccn1-c1ccccc1
C-C(=O)-[N;H0;D2;+0:1]=[c:2]1:[#16;a:3]:[c:4]:[c:5]:[#7;a:6]:1-[c:7]>>[NH;D1;+0:1]=[c:2]1:[#16;a:3]:[c:4]:[c:5]:[#7;a:6]:1-[c:7]
46.5
[{"value": 46.5, "product": "N=C1SC(=CN1C1=CC(=CC=C1)C(F)(F)F)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of 2-(acetylimino)-3-(3-trifluoromethylphenyl)-5-methylthiazoline (1 g) and hydrochloric acid (38 %, 4 ml) in ethanol-water (1:2, 15 ml) was refluxed for 3 hours. Ethanol was removed by distillation under reduced pressure, and the residue was neutralized with potassium carbonate, extracted with ethyl acetate ...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
c1cscn1.c1ccccc1
HO-
C(C)O.O
null
null
CC(=O)N=c1sc(C)cn1-c1cccc(C(F)(F)F)c1>C(C)O.O>Cc1cn(-c2cccc(C(F)(F)F)c2)c(=N)s1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-c55f62cea29848c7bf7668db86abb1e9
CCOC(=O)N=c1sc(Br)cn1-c1cccc(C(F)(F)F)c1>>CCOC(=O)N=c1sccn1-c1cccc(C(F)(F)F)c1
C(C)OC(=O)N=C1SC(=CN1C1=CC(=CC=C1)C(F)(F)F)Br.C(CCC)[SnH](CCCC)CCCC.C(C1=CC=CC=C1)(=O)OOC(C1=CC=CC=C1)=O>>C(C)OC(=O)N=C1SC=CN1C1=CC(=CC=C1)C(F)(F)F
Br[c:9]1[s:8][c:7](=[N:6][C:4]([O:3][CH2:2][CH3:1])=[O:5])[n:11](-[c:12]2[cH:13][cH:14][cH:15][c:16]([C:17]([F:18])([F:19])[F:20])[cH:21]2)[cH:10]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[N:6]=[c:7]1[s:8][cH:9][cH:10][n:11]1-[c:12]1[cH:13][cH:14][cH:15][c:16]([C:17]([F:18])([F:19])[F:20])[cH:21]1
CCOC(=O)N=c1sc(Br)cn1-c1cccc(C(F)(F)F)c1
CCOC(=O)N=c1sccn1-c1cccc(C(F)(F)F)c1
null
null
O1CCCC1
Functional Group Interconversion
Aromatic dehalogenation
4f6106989807e1170e2da8f2e1925119dcd1a22ece2cb0c7a904100c5bae54f5
56de34d4a44cb25d9380269ee5e138b0f24b40a3a0db22c5508049dc775a861f
N=c1sccn1-c1ccccc1
Br-[c;H0;D3;+0:1]1:[#16;a:2]:[c:3]:[#7;a:4](-[c:5]):[c:6]:1>>[c:5]-[#7;a:4]1:[c:6]:[cH;D2;+0:1]:[#16;a:2]:[c:3]:1
75.8
[{"value": 75.8, "product": "C(C)OC(=O)N=C1SC=CN1C1=CC(=CC=C1)C(F)(F)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 2-ethoxycarbonylimino-3-(3-trifluoromethylphenyl)-5-bromothiazoline (4.7 g), tributyltin hydride (6.9 g) and a catalytic amount of benzoyl peroxide in tetrahydrofuran (100 ml) was refluxed for 10 hours. The solvent was removed by distillation, and the residue was washed with hexane. Recrystallization from...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1cscn1
c1cscn1
c1cscn1.c1ccccc1
Br-
O1CCCC1
null
null
CCOC(=O)N=c1sc(Br)cn1-c1cccc(C(F)(F)F)c1>O1CCCC1>CCOC(=O)N=c1sccn1-c1cccc(C(F)(F)F)c1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-03cf8a9450bf45e38bbedbaf7ee743f1
CC=CCN(C(=S)NC(=O)OCC)c1cccc(C(F)(F)F)c1>>CC=CCN(C(N)=S)c1cccc(C(F)(F)F)c1
C(C=CC)N(C(=S)NC(=O)OCC)C1=CC(=CC=C1)C(F)(F)F.C[O-].[Na+]>>C(C=CC)N(C(=S)N)C1=CC(=CC=C1)C(F)(F)F
CCOC(=O)[NH:7][C:6]([N:5]([CH2:4][CH:3]=[CH:2][CH3:1])[c:9]1[cH:10][cH:11][cH:12][c:13]([C:14]([F:15])([F:16])[F:17])[cH:18]1)=[S:8]>>[CH3:1][CH:2]=[CH:3][CH2:4][N:5]([C:6]([NH2:7])=[S:8])[c:9]1[cH:10][cH:11][cH:12][c:13]([C:14]([F:15])([F:16])[F:17])[cH:18]1
CC=CCN(C(=S)NC(=O)OCC)c1cccc(C(F)(F)F)c1
CC=CCN(C(N)=S)c1cccc(C(F)(F)F)c1
null
null
CO
Reduction
Hydrogenolysis of amides/imides/carbamates
594e00c7c96b76cceef88e84b84e3b15c8ccccf89b962b4acfdce59b315169f0
2fc6be7095b4a5f0c4afd24643297a35f2252040d56517b70efbfde0b1038b8a
c1ccccc1
C-C-O-C(=O)-[NH;D2;+0:1]-[C:2](=[S;D1;H0:3])-[#7:4](-[c:5])-[C:6]-[C:7]=[C:8]>>[C:8]=[C:7]-[C:6]-[#7:4](-[c:5])-[C:2](-[NH2;D1;+0:1])=[S;D1;H0:3]
50.5
[{"value": 50.5, "product": "C(C=CC)N(C(=S)N)C1=CC(=CC=C1)C(F)(F)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of N-crotyl-N-(3-trifluoromethylphenyl)-N'-ethoxycarbonylthiourea (6 g) and sodium methoxide (28 % methanolic solution; 6.6 g) in methanol (100 ml) was refluxed for 2 days. After removal of the solvent, the residue was extracted with chloroform, washed with water and dried over anhydrous magnesium sulfate. T...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Thiourea
Thiourea
null
null
c1ccccc1
HO-
CO
null
null
CC=CCN(C(=S)NC(=O)OCC)c1cccc(C(F)(F)F)c1>CO>CC=CCN(C(N)=S)c1cccc(C(F)(F)F)c1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-7abe0b247b3646b18c986acb76de854f
CC(Br)Br.NC(=S)Nc1cccc(C(F)(F)F)c1>>N=C1SCCN1c1cccc(C(F)(F)F)c1
FC(C=1C=C(C=CC1)NC(=S)N)(F)F.BrC(C)Br.C([O-])([O-])=O.[K+].[K+]>>N=C1SCCN1C1=CC(=CC=C1)C(F)(F)F
Br[CH:5](Br)[CH3:4].[NH2:1][C:2](=[S:3])[NH:6][c:7]1[cH:8][cH:9][cH:10][c:11]([C:12]([F:13])([F:14])[F:15])[cH:16]1>>[NH:1]=[C:2]1[S:3][CH2:4][CH2:5][N:6]1[c:7]1[cH:8][cH:9][cH:10][c:11]([C:12]([F:13])([F:14])[F:15])[cH:16]1
CC(Br)Br.NC(=S)Nc1cccc(C(F)(F)F)c1
N=C1SCCN1c1cccc(C(F)(F)F)c1
null
null
CC(=O)C
Protection
OtherReaction
8c754bee2a863613e7708520561d09055ee64cc3793115f8e576e60bae5af171
101460e55348dc63801d065e571f149bdadd19d7ea2f7cddc1402a217c094fa3
N=C1SCCN1c1ccccc1
Br-[CH;D3;+0:1](-Br)-[CH3;D1;+0:2].[NH2;D1;+0:3]-[C;H0;D3;+0:4](=[S;H0;D1;+0:5])-[NH;D2;+0:6]-[c:7](:[c:8]):[c:9]>>[NH;D1;+0:3]=[C;H0;D3;+0:4]1-[S;H0;D2;+0:5]-[CH2;D2;+0:2]-[CH2;D2;+0:1]-[N;H0;D3;+0:6]-1-[c:7](:[c:8]):[c:9]
110
[{"value": 110.0, "product": "N=C1SCCN1C1=CC(=CC=C1)C(F)(F)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of N-(3-trifluoromethylphenyl)thiourea (6.1 g), dibromoethane (5.7 g) and anhydrous potassium carbonate (11.5 g) in acetone (60 ml) was refluxed for 1 day. The solvent was removed by distillation therefrom, and the residue was extracted with ethyl ether, washed with water, dried over anhydrous magnesium sulf...
10.6084/m9.figshare.5104873.v1
null
Secondary halide.Secondary halide.Thiourea
Tertiary amine.Monosulfide
null
C1CSC[NH]1
C1CSC[NH]1.c1ccccc1
HBr
CC(=O)C
null
null
CC(Br)Br.NC(=S)Nc1cccc(C(F)(F)F)c1>CC(=O)C>N=C1SCCN1c1cccc(C(F)(F)F)c1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-2646e83101e44194b575c8e4dfed9fd9
CCCCOC(=O)Cl.N=C1SCCN1c1cccc(C(F)(F)F)c1>>CCCCOC(=O)N=C1SCCN1c1cccc(C(F)(F)F)c1
N=C1SCCN1C1=CC(=CC=C1)C(F)(F)F.C(OCCCC)(=O)Cl.C(C)N(CC)CC>>C(CCC)OC(=O)N=C1SCCN1C1=CC(=CC=C1)C(F)(F)F
Cl[C:6]([O:5][CH2:4][CH2:3][CH2:2][CH3:1])=[O:7].[NH:8]=[C:9]1[S:10][CH2:11][CH2:12][N:13]1[c:14]1[cH:15][cH:16][cH:17][c:18]([C:19]([F:20])([F:21])[F:22])[cH:23]1>>[CH3:1][CH2:2][CH2:3][CH2:4][O:5][C:6](=[O:7])[N:8]=[C:9]1[S:10][CH2:11][CH2:12][N:13]1[c:14]1[cH:15][cH:16][cH:17][c:18]([C:19]([F:20])([F:21])[F:22])[cH:...
CCCCOC(=O)Cl.N=C1SCCN1c1cccc(C(F)(F)F)c1
CCCCOC(=O)N=C1SCCN1c1cccc(C(F)(F)F)c1
null
null
O1CCCC1
Acylation
OtherReaction
f82c583524f79166411cb496627fa3c85d4aefc3413e305ade9275efe2428bc2
d03c43b1eb3e007d0a26c663cd0f6b51f594c27d1ade9616fb1640d35a60bddb
N=C1SCCN1c1ccccc1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[#8:3]-[C:4].[NH;D1;+0:5]=[C:6]1-[#16:7]-[C:8]-[C:9]-[#7:10]-1-[c:11]>>[C:4]-[#8:3]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[N;H0;D2;+0:5]=[C:6]1-[#16:7]-[C:8]-[C:9]-[#7:10]-1-[c:11]
40.5
[{"value": 40.5, "product": "C(CCC)OC(=O)N=C1SCCN1C1=CC(=CC=C1)C(F)(F)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of N-(3-trifluoromethylphenyl)thiourea (6.1 g), dibromoethane (5.7 g) and anhydrous potassium carbonate (11.5 g) in acetone (60 ml) was refluxed for 1 day. The solvent was removed by distillation therefrom, and the residue was extracted with ethyl ether, washed with water, dried over anhydrous magnesium sulf...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Ether
Ether
null
null
C1CSC[NH]1.c1ccccc1
HCl
O1CCCC1
null
null
CCCCOC(=O)Cl.N=C1SCCN1c1cccc(C(F)(F)F)c1>O1CCCC1>CCCCOC(=O)N=C1SCCN1c1cccc(C(F)(F)F)c1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-fa8d09f785da43d08f3fafc57bc6778e
CC(Br)Br.CCOC(=O)NC(=S)Nc1cccc(C(F)(F)F)c1>>CCOC(=O)N=C1SCCN1c1cccc(C(F)(F)F)c1
FC(C=1C=C(C=CC1)NC(=S)NC(=O)OCC)(F)F.BrC(C)Br.C([O-])([O-])=O.[K+].[K+]>>C(C)OC(=O)N=C1SCCN1C1=CC(=CC=C1)C(F)(F)F
Br[CH:10](Br)[CH3:9].[CH3:1][CH2:2][O:3][C:4](=[O:5])[NH:6][C:7](=[S:8])[NH:11][c:12]1[cH:13][cH:14][cH:15][c:16]([C:17]([F:18])([F:19])[F:20])[cH:21]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[N:6]=[C:7]1[S:8][CH2:9][CH2:10][N:11]1[c:12]1[cH:13][cH:14][cH:15][c:16]([C:17]([F:18])([F:19])[F:20])[cH:21]1
CC(Br)Br.CCOC(=O)NC(=S)Nc1cccc(C(F)(F)F)c1
CCOC(=O)N=C1SCCN1c1cccc(C(F)(F)F)c1
null
null
CC(=O)C
Protection
OtherReaction
d6f618ec53b6862d1ff2960c4e6a2b010fc7d1f3fee77a86188252744c890acc
6f23c5b879e9820f6e48620bc2d18d56d8fa8f76fe736e09f5876deb392a7395
N=C1SCCN1c1ccccc1
Br-[CH;D3;+0:1](-Br)-[CH3;D1;+0:2].[C:3]-[#8:4]-[C:5](=[O;D1;H0:6])-[NH;D2;+0:7]-[C;H0;D3;+0:8](=[S;H0;D1;+0:9])-[NH;D2;+0:10]-[c:11](:[c:12]):[c:13]>>[C:3]-[#8:4]-[C:5](=[O;D1;H0:6])-[N;H0;D2;+0:7]=[C;H0;D3;+0:8]1-[S;H0;D2;+0:9]-[CH2;D2;+0:2]-[CH2;D2;+0:1]-[N;H0;D3;+0:10]-1-[c:11](:[c:12]):[c:13]
83.1
[{"value": 83.1, "product": "C(C)OC(=O)N=C1SCCN1C1=CC(=CC=C1)C(F)(F)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of N-(3-trifluoromethylphenyl)-N'-ethoxycarbonylthiourea (1.8 g), dibromoethane (1.29 g) and anhydrous potassium carbonate (2.6 g) in acetone (20 ml) was refluxed for 5 hours. The solvent was removed by distillation, and the residue was extracted with diethyl ether. The extract was washed with water, dried o...
10.6084/m9.figshare.5104873.v1
null
Secondary halide.Secondary halide.Carbamic ester.Thiourea
Tertiary amine.Monosulfide
null
C1CSC[NH]1
C1CSC[NH]1.c1ccccc1
HBr
CC(=O)C
null
null
CC(Br)Br.CCOC(=O)NC(=S)Nc1cccc(C(F)(F)F)c1>CC(=O)C>CCOC(=O)N=C1SCCN1c1cccc(C(F)(F)F)c1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-05aff642a9524aeeb782b83184544cc8
CC(C)C(C)(N)C(N)=O.CCOC(=O)c1cnc(C)nc1C(=O)OCC>>Cc1ncc(C(=O)O)c(C2=NC(C)(C(C)C)C(=O)N2)n1
CC1=NC=C(C(=N1)C(=O)OCC)C(=O)OCC.NC(C(=O)N)(C(C)C)C>>CC1=NC=C(C(=N1)C=1NC(C(N1)(C(C)C)C)=O)C(=O)O
[NH2:11][C:12]([CH3:13])([CH:14]([CH3:15])[CH3:16])[C:17](=[O:18])[NH2:19].CCO[C:10](=O)[c:9]1[c:5]([C:6](=[O:7])[O:8]CC)[cH:4][n:3][c:2]([CH3:1])[n:20]1>>[CH3:1][c:2]1[n:3][cH:4][c:5]([C:6](=[O:7])[OH:8])[c:9]([C:10]2=[N:11][C:12]([CH3:13])([CH:14]([CH3:15])[CH3:16])[C:17](=[O:18])[NH:19]2)[n:20]1
CC(C)C(C)(N)C(N)=O.CCOC(=O)c1cnc(C)nc1C(=O)OCC
Cc1ncc(C(=O)O)c(C2=NC(C)(C(C)C)C(=O)N2)n1
null
null
C1(=CC=CC=C1)C
Heteroatom Alkylation and Arylation
OtherReaction
3b698ee4f54c66f1d46998658008290900266bbd2feba49593a4d93a59594863
eb44f496e8f1313af2c0f91b3e3b1cbaaa1a96970b8e4c17561608a8e6dd9f5a
O=C1CN=C(c2ccncn2)N1
C-C-O-[C;H0;D3;+0:1](=O)-[c:2]1:[#7;a:3]:[c:4]:[#7;a:5]:[c:6]:[c:7]:1-[C:8](=[O;D1;H0:9])-[O;H0;D2;+0:10]-C-C.[C:11]-[C:12](-[C;D1;H3:13])(-[NH2;D1;+0:14])-[C:15](-[NH2;D1;+0:16])=[O;D1;H0:17]>>[C:11]-[C:12]1(-[C;D1;H3:13])-[N;H0;D2;+0:14]=[C;H0;D3;+0:1](-[c:2]2:[#7;a:3]:[c:4]:[#7;a:5]:[c:6]:[c:7]:2-[C:8](=[O;D1;H0:9])...
51.5
[{"value": 51.0, "product": "CC1=NC=C(C(=N1)C=1NC(C(N1)(C(C)C)C)=O)C(=O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 51.5, "product": "CC1=NC=C(C(=N1)C=1NC(C(N1)(C(C)C)C)=O)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
16
HOUR
To a mixture of 98.8 g (0.415 mole) of diethyl 2-methylpyrimidine-4,5-dicarboxylate (compare, for example, J. Heterocycl. Chem. 2, 202-204 [1965]) and 54.0 g (0.415 mole) of 2-amino-2,3-dimethylbutyramide in 700 ml of anhydrous toluene there are added in portions 102.2 g (0.913 mole) of potassium tert.-butylate, and th...
10.6084/m9.figshare.5104873.v1
null
Ester.Ester.Primary amide.Primary amine
Carboxylic acid.Secondary amide
null
C1=NCCN1
c1cncnc1.C1=NCCN1
HO-
C1(=CC=CC=C1)C
80
16
CC(C)C(C)(N)C(N)=O.CCOC(=O)c1cnc(C)nc1C(=O)OCC>C1(=CC=CC=C1)C>Cc1ncc(C(=O)O)c(C2=NC(C)(C(C)C)C(=O)N2)n1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-cac5b60f283041dda7c7abbd2044a9b6
CCOC(=O)c1nc(SC)sc1C(=O)OCC>>CCOC(=O)c1nc(SC)sc1C(=O)O
[OH-].[Na+].CSC=1SC(=C(N1)C(=O)OCC)C(=O)OCC>>C(C)OC(=O)C=1N=C(SC1C(=O)O)SC
CC[O:15][C:13]([c:12]1[c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[n:7][c:8]([S:9][CH3:10])[s:11]1)=[O:14]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[n:7][c:8]([S:9][CH3:10])[s:11][c:12]1[C:13](=[O:14])[OH:15]
CCOC(=O)c1nc(SC)sc1C(=O)OCC
CCOC(=O)c1nc(SC)sc1C(=O)O
null
null
O.C(C)O.O
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1cscn1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4](:[#16;a:5]):[c:6]:[#7;a:7]>>[#16;a:5]:[c:4](-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]):[c:6]:[#7;a:7]
null
[]
null
null
1
HOUR
At room temperature, a solution of 1.10 g (27.5 mmol) of sodium hydroxide in 10 ml of water was added over a period of one hour to a solution of 7.00 g (25 mmol) of diethyl 2-methylthiothiazole-4,5-dicarboxylate in 100 ml of ethanol/water (2:1). The mixture was stirred for one hour, the solvent mixture was then removed...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1cscn1
Other
O.C(C)O.O
null
1
CCOC(=O)c1nc(SC)sc1C(=O)OCC>O.C(C)O.O>CCOC(=O)c1nc(SC)sc1C(=O)O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-c86211829d6b4c1584a76548e6ee953b
CC(C)(C)NC(=O)c1csc(Br)n1.C[O-]>>COc1nc(C(=O)NC(C)(C)C)cs1
C[O-].[Na+].C(C)(C)(C)NC(=O)C=1N=C(SC1)Br>>C(C)(C)(C)NC(=O)C=1N=C(SC1)OC
Br[c:3]1[n:4][c:5]([C:6](=[O:7])[NH:8][C:9]([CH3:10])([CH3:11])[CH3:12])[cH:13][s:14]1.[CH3:1][O-:2]>>[CH3:1][O:2][c:3]1[n:4][c:5]([C:6](=[O:7])[NH:8][C:9]([CH3:10])([CH3:11])[CH3:12])[cH:13][s:14]1
CC(C)(C)NC(=O)c1csc(Br)n1.C[O-]
COc1nc(C(=O)NC(C)(C)C)cs1
null
null
CO
Heteroatom Alkylation and Arylation
OtherReaction
361dd26d5fe71f37e48dfadda08834dc24dbeb11757b91bcc09fe7edbef36ae1
51fd03eb6a688046e417b9ed09ea0e72062396d005af1318b9b5f376a97da959
c1cscn1
Br-[c;H0;D3;+0:1]1:[#16;a:2]:[c:3]:[c:4](-[C:5](-[#7:6])=[O;D1;H0:7]):[#7;a:8]:1.[C;D1;H3:9]-[O-;H0;D1:10]>>[#7:6]-[C:5](=[O;D1;H0:7])-[c:4]1:[#7;a:8]:[c;H0;D3;+0:1](-[O;H0;D2;+0:10]-[C;D1;H3:9]):[#16;a:2]:[c:3]:1
98
[{"value": 98.0, "product": "C(C)(C)(C)NC(=O)C=1N=C(SC1)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 97.4, "product": "C(C)(C)(C)NC(=O)C=1N=C(SC1)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
At 25° C., 8.90 g of a 30% strength solution (49 mmol) of sodium methanolate in methanol was added to a solution of 12.00 g (46 mmol) of 2-bromothiazole-4-carboxylic acid-tert.-butylamide in 150 ml of methanol. The mixture was boiled under reflux for four hours, the clear solution was evaporated down, the residue was t...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
Ether
c1cscn1
c1cscn1
c1cscn1
Br-
CO
null
null
CC(C)(C)NC(=O)c1csc(Br)n1.C[O-]>CO>COc1nc(C(=O)NC(C)(C)C)cs1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-7521a5ff0c9d4c75bde504a8fa790722
CC(C)c1nc(C(=O)O)co1.NC1CC1>>CC(C)c1nc(C(=O)NC2CC2)co1
S(=O)(Cl)Cl.C1(CC1)N.O.C(C)(C)C=1OC=C(N1)C(=O)O>>C1(CC1)NC(=O)C=1N=C(OC1)C(C)C
O[C:7]([c:6]1[n:5][c:4]([CH:2]([CH3:1])[CH3:3])[o:14][cH:13]1)=[O:8].[NH2:9][CH:10]1[CH2:11][CH2:12]1>>[CH3:1][CH:2]([CH3:3])[c:4]1[n:5][c:6]([C:7](=[O:8])[NH:9][CH:10]2[CH2:11][CH2:12]2)[cH:13][o:14]1
CC(C)c1nc(C(=O)O)co1.NC1CC1
CC(C)c1nc(C(=O)NC2CC2)co1
null
null
CN(C=O)C.C1(=CC=CC=C1)C.ClCCl
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(NC1CC1)c1cocn1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#7;a:4]:[c:5]:[#8;a:6]:[c:7]:1.[NH2;D1;+0:8]-[C:9]1-[C:10]-[C:11]-1>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:8]-[C:9]1-[C:10]-[C:11]-1)-[c:3]1:[#7;a:4]:[c:5]:[#8;a:6]:[c:7]:1
96
[{"value": 96.0, "product": "C1(CC1)NC(=O)C=1N=C(OC1)C(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 95.8, "product": "C1(CC1)NC(=O)C=1N=C(OC1)C(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
1
HOUR
At room temperature, 47.6 g (0.40 mol) of thionyl chloride was dripped into a solution of 31.0 g (0.20 mol) of 2-isopropyloxazole-4-carboxylic acid in 200 ml of toluene and 2 ml of dimethylformamide, and the mixture was stirred for one hour at 80° C. The solvents were stripped off under reduced pressure, the residue wa...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1cocn1.C1CC1
HO-
CN(C=O)C.C1(=CC=CC=C1)C.ClCCl
80
1
CC(C)c1nc(C(=O)O)co1.NC1CC1>CN(C=O)C.C1(=CC=CC=C1)C.ClCCl>CC(C)c1nc(C(=O)NC2CC2)co1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-6db241b1de6942798489126e4163fdde
CC(C)c1nc(C(=O)NC2CC2)co1.O=C=O>>CC(C)c1nc(C(=O)NC2CC2)c(C(=O)O)o1
C(=O)=O.C(CCC)[Li].C1(CC1)NC(=O)C=1N=C(OC1)C(C)C>>C1(CC1)NC(=O)C=1N=C(OC1C(=O)O)C(C)C
[CH3:1][CH:2]([CH3:3])[c:4]1[n:5][c:6]([C:7](=[O:8])[NH:9][CH:10]2[CH2:11][CH2:12]2)[cH:13][o:17]1.[C:14](=[O:15])=[O:16]>>[CH3:1][CH:2]([CH3:3])[c:4]1[n:5][c:6]([C:7](=[O:8])[NH:9][CH:10]2[CH2:11][CH2:12]2)[c:13]([C:14](=[O:15])[OH:16])[o:17]1
CC(C)c1nc(C(=O)NC2CC2)co1.O=C=O
CC(C)c1nc(C(=O)NC2CC2)c(C(=O)O)o1
null
null
CCCCCC.O1CCCC1
Acylation
OtherReaction
d7009895e441ce741d63fde0f10b8e58aef3dda277984d0da32c335724def808
f2fa2063dd26da08ea200eb6cbb3037b91013a82352a2b60120e98f9e54cbd88
O=C(NC1CC1)c1cocn1
[C:1]-[#7:2]-[C:3](=[O;D1;H0:4])-[c:5]1:[#7;a:6]:[c:7](-[C:8]):[#8;a:9]:[cH;D2;+0:10]:1.[O;D1;H0:11]=[C;H0;D2;+0:12]=[O;H0;D1;+0:13]>>[C:1]-[#7:2]-[C:3](=[O;D1;H0:4])-[c:5]1:[#7;a:6]:[c:7](-[C:8]):[#8;a:9]:[c;H0;D3;+0:10]:1-[C;H0;D3;+0:12](=[O;D1;H0:11])-[OH;D1;+0:13]
81
[{"value": 81.0, "product": "C1(CC1)NC(=O)C=1N=C(OC1C(=O)O)C(C)C", "details": "PERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
At -70° C. and under a nitrogen blanket, 0.12 mol of n-butyllithium (80.0 ml of a 1.5 molar solution in hexane) was dripped into a solution of 10.4 g (0.054 mol) of 2-isopropyloxazole-4-carboxylic acid-cyclopropylamide in 250 ml of tetrahydrofuran, and the mixture was stirred for 30 minutes at this temperature. The rea...
10.6084/m9.figshare.5104873.v1
null
Carbon dioxide
Carboxylic acid
c1cocn1
c1cocn1
c1cocn1.C1CC1
null
CCCCCC.O1CCCC1
null
0.5
CC(C)c1nc(C(=O)NC2CC2)co1.O=C=O>CCCCCC.O1CCCC1>CC(C)c1nc(C(=O)NC2CC2)c(C(=O)O)o1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-e8d6c976acfe418eb1c313ed305dfb2d
CC(C)(C)N.CCOC(=O)c1nc(SC)sc1C(=O)Cl>>CCOC(=O)c1nc(SC)sc1C(=O)NC(C)(C)C
C(C)OC(=O)C=1N=C(SC1C(=O)Cl)SC.C(C)(C)(C)N.Cl>>C(C)(C)(C)NC(=O)C1=C(N=C(S1)SC)C(=O)OCC
[NH2:15][C:16]([CH3:17])([CH3:18])[CH3:19].Cl[C:13]([c:12]1[c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[n:7][c:8]([S:9][CH3:10])[s:11]1)=[O:14]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[n:7][c:8]([S:9][CH3:10])[s:11][c:12]1[C:13](=[O:14])[NH:15][C:16]([CH3:17])([CH3:18])[CH3:19]
CC(C)(C)N.CCOC(=O)c1nc(SC)sc1C(=O)Cl
CCOC(=O)c1nc(SC)sc1C(=O)NC(C)(C)C
null
null
ClCCl
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
c1cscn1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#16;a:4]:[c:5]:[#7;a:6]:[c:7]:1-[C:8](-[#8:9])=[O;D1;H0:10].[C;D1;H3:11]-[C:12](-[C;D1;H3:13])(-[C;D1;H3:14])-[NH2;D1;+0:15]>>[#8:9]-[C:8](=[O;D1;H0:10])-[c:7]1:[#7;a:6]:[c:5]:[#16;a:4]:[c:3]:1-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:15]-[C:12](-[C;D1;H3:11])(-[C;D1;H3:13])-[C;D1;...
100.2
[{"value": 100.0, "product": "C(C)(C)(C)NC(=O)C1=C(N=C(S1)SC)C(=O)OCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 100.2, "product": "C(C)(C)(C)NC(=O)C1=C(N=C(S1)SC)C(=O)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
14
HOUR
3.50 g (13.2 mmol) of 4-ethoxycarbonyl-2-methylthiothiazole-5-carboxylic acid chloride was dissolved in 20 ml of dichloromethane and dripped, at 0° C., into a solution of 3.20 g (44 mmol) of tert-butylamine in 50 ml of dichloromethane. The mixture was allowed to warm up to room temperature and was then stirred for 14 h...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1cscn1
HCl
ClCCl
null
14
CC(C)(C)N.CCOC(=O)c1nc(SC)sc1C(=O)Cl>ClCCl>CCOC(=O)c1nc(SC)sc1C(=O)NC(C)(C)C
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-2edd7bfaf0f643ea9042f3b3d6c043f5
CCOC(=O)c1nc(SC)sc1C(=O)NC(C)(C)C>>CSc1nc(C(=O)O)c(C(=O)NC(C)(C)C)s1
[OH-].[K+].C(C)(C)(C)NC(=O)C1=C(N=C(S1)SC)C(=O)OCC>>C(C)(C)(C)NC(=O)C1=C(N=C(S1)SC)C(=O)O
CC[O:8][C:6]([c:5]1[n:4][c:3]([S:2][CH3:1])[s:17][c:9]1[C:10](=[O:11])[NH:12][C:13]([CH3:14])([CH3:15])[CH3:16])=[O:7]>>[CH3:1][S:2][c:3]1[n:4][c:5]([C:6](=[O:7])[OH:8])[c:9]([C:10](=[O:11])[NH:12][C:13]([CH3:14])([CH3:15])[CH3:16])[s:17]1
CCOC(=O)c1nc(SC)sc1C(=O)NC(C)(C)C
CSc1nc(C(=O)O)c(C(=O)NC(C)(C)C)s1
null
null
O.C(C)O.O
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1cscn1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4](:[#7;a:5]):[c:6]:[#16;a:7]>>[#16;a:7]:[c:6]:[c:4](-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]):[#7;a:5]
null
[]
null
null
null
null
0.82 g (14.6 mmol) of potassium hydroxide in 10 ml of water was added to a solution of 4.00 g (13.2 mmol) of 4-ethoxycarbonyl-2-methylthiothiazole-5-carboxylic acid-tert-butylamide in 50 ml of water/ethanol (2:1), and the mixture was refluxed for 2 hours. The solvent mixture was then removed under reduced pressure and ...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1cscn1
Other
O.C(C)O.O
null
null
CCOC(=O)c1nc(SC)sc1C(=O)NC(C)(C)C>O.C(C)O.O>CSc1nc(C(=O)O)c(C(=O)NC(C)(C)C)s1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-918dffba71544237accb80156ad6bdb6
C=O.CC(C)C[C@H](N)C(=O)O.CC(C)C[C@H](NC(=O)OC(C)(C)C)C(=O)O>>CC(C)(C)OC(=O)N[C@@H](Cc1cc2ccccc2[nH]1)C(=O)O.CC(C)C[C@@H](C=O)NC(=O)OC(C)(C)C.CC(C)C[C@H](NC(=O)OC(C)(C)C)C(=O)O
N([C@@H](CC(C)C)C(=O)O)C(=O)OC(C)(C)C.C=O.N[C@@H](CC(C)C)C(=O)O>>N([C@@H](CC(C)C)C(=O)O)C(=O)OC(C)(C)C.CC(C)(C)OC(=O)N[C@@H](CC1=CC=2C=CC=CC2N1)C(=O)O.N([C@@H](CC(C)C)C=O)C(=O)OC(C)(C)C
[O:5]=[CH2:6].[NH2:8][C@H:9]([C:20](=[O:21])[OH:22])[CH2:26][CH:24]([CH3:15])[CH3:25].[CH3:1][C:47]([CH3:2])([CH3:37])[O:46][C:44]([NH:43][C@@H:42]([CH2:41][CH:39]([CH3:38])[CH3:40])[C:51](=[O:52])[OH:53])=[O:45]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[NH:8][C@@H:9]([CH2:10][c:11]1[cH:12][c:13]2[cH:14][cH:15]...
C=O.CC(C)C[C@H](N)C(=O)O.CC(C)C[C@H](NC(=O)OC(C)(C)C)C(=O)O
CC(C)(C)OC(=O)N[C@@H](Cc1cc2ccccc2[nH]1)C(=O)O.CC(C)C[C@@H](C=O)NC(=O)OC(C)(C)C.CC(C)C[C@H](NC(=O)OC(C)(C)C)C(=O)O
null
null
null
Aromatic Heterocycle Formation
OtherReaction
2ffa72b2b656fefbc22f8e826b951442ec3c478a39284e3074cd512611ac0f4b
8cbc1340892c80b218777bc6c951083673d7f43dbdc033f7e1a13d0cd1c5623b
c1ccc2[nH]ccc2c1
[#7:1]-[C:2](=[O;D1;H0:3])-[#8:4]-[C;H0;D4;+0:5](-[CH3;D1;+0:6])(-[CH3;D1;+0:7])-[CH3;D1;+0:8].[C;D1;H3:9]-[CH;D3;+0:10](-[CH3;D1;+0:11])-[CH2;D2;+0:12]-[C@H;D3;+0:13](-[NH2;D1;+0:14])-[C:15](=[O;D1;H0:16])-[O;D1;H1:17].[CH2;D1;+0:18]=[O;H0;D1;+0:19]>>[#7:20]-[C:21](-[C:22])-[CH2;D2;+0:12]-[CH;D3;+0:10](-[C;D1;H3:23])-...
null
[]
null
null
null
null
Leu-psi -Tpi-BHA resin is made by reacting Boc-Leu-psi -Trp-BHA resin with formaldehyde in accordance with the procedures as follows: Boc-Leu-psi -Trp-BHA resin is obtained from 1.0 g BHA resin (0.9 m mode NH2 g) with coupling Boc-Trp and Boc-Leu-CHO successively by the method indicated in Operation I and Operation II....
10.6084/m9.figshare.5104873.v1
null
Formaldehyde.Ether.Primary amine.Boc
Aldehyde.Carbamic ester.Carbamic ester.Ether.Ether.Ether.Boc.Boc.Boc
null
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1
Other
null
null
null
C=O.CC(C)C[C@H](N)C(=O)O.CC(C)C[C@H](NC(=O)OC(C)(C)C)C(=O)O>>CC(C)(C)OC(=O)N[C@@H](Cc1cc2ccccc2[nH]1)C(=O)O.CC(C)C[C@@H](C=O)NC(=O)OC(C)(C)C.CC(C)C[C@H](NC(=O)OC(C)(C)C)C(=O)O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-da46530a89434c3c8d249230d0da1142
CCCC[C@H](NC(=O)OC(C)(C)C)C(=O)N1CCC[C@H]1C(N)=O>>CCCC[C@H](N)C(=O)N1CCC[C@H]1C(N)=O
C(C)(C)(C)OC(=O)N[C@@H](CCCC)C(=O)N1[C@H](C(=O)N)CCC1.Cl.O1CCOCC1>>Cl.N[C@@H](CCCC)C(=O)N1[C@H](C(=O)N)CCC1
CC(C)(C)OC(=O)[NH:6][C@@H:5]([CH2:4][CH2:3][CH2:2][CH3:1])[C:7](=[O:8])[N:9]1[CH2:10][CH2:11][CH2:12][C@H:13]1[C:14]([NH2:15])=[O:16]>>[CH3:1][CH2:2][CH2:3][CH2:4][C@H:5]([NH2:6])[C:7](=[O:8])[N:9]1[CH2:10][CH2:11][CH2:12][C@H:13]1[C:14]([NH2:15])=[O:16]
CCCC[C@H](NC(=O)OC(C)(C)C)C(=O)N1CCC[C@H]1C(N)=O
CCCC[C@H](N)C(=O)N1CCC[C@H]1C(N)=O
null
null
null
Reduction
Hydrogenolysis of amides/imides/carbamates
3c33dd2a2d355ee5ba0287367e209aa147a39aa00607f0c95fb2bf1ade45d014
c5b5dffe7dd8beebdc1baa8b5b05300a9f7079e65dcfd42ade6f8a77ff09537d
C1CCNC1
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[C:2](-[C:3])-[C:4](=[O;D1;H0:5])-[#7:6](-[C:7])-[C:8]-[C:9](-[N;D1;H2:10])=[O;D1;H0:11]>>[C:7]-[#7:6](-[C:4](=[O;D1;H0:5])-[C:2](-[C:3])-[NH2;D1;+0:1])-[C:8]-[C:9](-[N;D1;H2:10])=[O;D1;H0:11]
95
[{"value": 95.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
The N-tert-butyloxycarbonyl-L-norleucyl-proline amide (1 g, 3.05 mmol) was placed in a round bottom flask to which freshly prepared 4N HCl/dioxane (25 ml) was added. The solution was stirred for 1 hour. Evaporation of solvent in vacuo and then crystallization of an oily residue from methanol/ethyl ether gave the title ...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Boc
Primary amine
null
null
C1CC[NH]C1
HO-
null
null
1
CCCC[C@H](NC(=O)OC(C)(C)C)C(=O)N1CCC[C@H]1C(N)=O>>CCCC[C@H](N)C(=O)N1CCC[C@H]1C(N)=O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-0d244421dc454fa580394fccb09e3665
Nc1ccccc1.O=C(Cl)c1cc2ccccc2s1>>O=C(Nc1ccccc1)c1cc2ccccc2s1
S1C(=CC2=C1C=CC=C2)C(=O)Cl.NC1=CC=CC=C1.O>>S1C(=CC2=C1C=CC=C2)C(=O)NC2=CC=CC=C2
[NH2:3][c:4]1[cH:5][cH:6][cH:7][cH:8][cH:9]1.Cl[C:2](=[O:1])[c:10]1[cH:11][c:12]2[cH:13][cH:14][cH:15][cH:16][c:17]2[s:18]1>>[O:1]=[C:2]([NH:3][c:4]1[cH:5][cH:6][cH:7][cH:8][cH:9]1)[c:10]1[cH:11][c:12]2[cH:13][cH:14][cH:15][cH:16][c:17]2[s:18]1
Nc1ccccc1.O=C(Cl)c1cc2ccccc2s1
O=C(Nc1ccccc1)c1cc2ccccc2s1
null
null
C1(=CC=CC=C1)C
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
O=C(Nc1ccccc1)c1cc2ccccc2s1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[#16;a:5]:[c:6].[NH2;D1;+0:7]-[c:8](:[c:9]):[c:10]>>[O;D1;H0:2]=[C;H0;D3;+0:1](-[NH;D2;+0:7]-[c:8](:[c:9]):[c:10])-[c:3](:[c:4]):[#16;a:5]:[c:6]
77
[{"value": 77.0, "product": "S1C(=CC2=C1C=CC=C2)C(=O)NC2=CC=CC=C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 76.6, "product": "S1C(=CC2=C1C=CC=C2)C(=O)NC2=CC=CC=C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
50
CELSIUS
5
HOUR
To 8 g (0.0407 mol) of benzothiophene-2-carboxylic acid chloride in 150 ml of toluene there are added with stirring at room temperature 7.6 g (0.0814 mol) of anilin, then, when the addition is complete, the mixture is stirred for 5 hours at 50° C., the reaction mixture is then poured into water, and precipitate which h...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1ccccc1.c1ccc2sccc2c1
HCl
C1(=CC=CC=C1)C
50
5
Nc1ccccc1.O=C(Cl)c1cc2ccccc2s1>C1(=CC=CC=C1)C>O=C(Nc1ccccc1)c1cc2ccccc2s1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-5496bc558f464336aaaccae32ef16785
CC(=O)c1ccc([C@H]2C[C@@]3(C)[C@H](CC[C@]3(O)CC#C[Si](C)(C)C)[C@@H]3CCC4=CC(=O)CCC4=C32)cc1>>C#CC[C@@]1(O)CC[C@@H]2[C@@H]3CCC4=CC(=O)CCC4=C3[C@@H](c3ccc(C(C)=O)cc3)C[C@@]21C
C(C)(=O)C1=CC=C(C=C1)[C@@H]1C2=C3CCC(C=C3CC[C@H]2[C@H]2CC[C@@]([C@@]2(C)C1)(CC#C[Si](C)(C)C)O)=O.[F-].C(CCC)[N+](CCCC)(CCCC)CCCC>>C(C)(=O)C1=CC=C(C=C1)[C@@H]1C2=C3CCC(C=C3CC[C@H]2[C@H]2CC[C@@]([C@@]2(C)C1)(CC#C)O)=O
C[Si](C)(C)[C:1]#[C:2][CH2:3][C@@:4]1([OH:5])[CH2:6][CH2:7][C@@H:8]2[C@@H:9]3[CH2:10][CH2:11][C:12]4=[CH:13][C:14](=[O:15])[CH2:16][CH2:17][C:18]4=[C:19]3[C@@H:20]([c:21]3[cH:22][cH:23][c:24]([C:25]([CH3:26])=[O:27])[cH:28][cH:29]3)[CH2:30][C@:31]12[CH3:32]>>[CH:1]#[C:2][CH2:3][C@@:4]1([OH:5])[CH2:6][CH2:7][C@@H:8]2[C@...
CC(=O)c1ccc([C@H]2C[C@@]3(C)[C@H](CC[C@]3(O)CC#C[Si](C)(C)C)[C@@H]3CCC4=CC(=O)CCC4=C32)cc1
C#CC[C@@]1(O)CC[C@@H]2[C@@H]3CCC4=CC(=O)CCC4=C3[C@@H](c3ccc(C(C)=O)cc3)C[C@@]21C
null
null
O1CCCC1
Deprotection
TMS deprotection from alkyne
e85676bb81da384790c9c858d44f182cdd01e3a79f77f7a239fe38487234cb96
56d526d7c9cb1bd7bee4940e216a9b1dd4597fd025a186b8d6e4675d8f4db26b
O=C1C=C2CC[C@@H]3C(=C2CC1)[C@@H](c1ccccc1)CC1CCC[C@@H]13
C-[Si](-C)(-C)-[C;H0;D2;+0:1]#[C:2]-[C:3]>>[C:3]-[C:2]#[CH;D1;+0:1]
69.6
[{"value": 69.6, "product": "C(C)(=O)C1=CC=C(C=C1)[C@@H]1C2=C3CCC(C=C3CC[C@H]2[C@H]2CC[C@@]([C@@]2(C)C1)(CC#C)O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
5
MINUTE
470 mg of 11beta-(4-Acetylphenyl)-17alpha-hydroxy-17-(3-trimethysilyl-2-propinyl)-14beta-estra-4,9-dien-3-one in 24 ml of tetrahydrofuran is mixed with 2.35 ml of a 1M solution of tetrabutylammonium fluoride in tetrahydrofuran and stirred for 5 minutes at room temperature. It is poured on water and extracted with ethyl...
10.6084/m9.figshare.5104873.v1
null
Alkyne.Silyl protective group
Alkyne
null
null
c1ccccc1.C1=C2CC[C@@H]3C(=C2CCC1)CC[C@@H]1CCC[C@@H]13
Other
O1CCCC1
null
0.083333
CC(=O)c1ccc([C@H]2C[C@@]3(C)[C@H](CC[C@]3(O)CC#C[Si](C)(C)C)[C@@H]3CCC4=CC(=O)CCC4=C32)cc1>O1CCCC1>C#CC[C@@]1(O)CC[C@@H]2[C@@H]3CCC4=CC(=O)CCC4=C3[C@@H](c3ccc(C(C)=O)cc3)C[C@@]21C
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-7844a06e09664a17934167953fba756b
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1cccnc1.Oc1ccc(Br)cc1>>Oc1ccc(-c2cccnc2)cc1
BrC1=CC=C(C=C1)O.C(CCC)[Sn](C=1C=NC=CC1)(CCCC)CCCC>>N1=CC(=CC=C1)C1=CC=C(C=C1)O
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c:6]1[cH:7][cH:8][cH:9][n:10][cH:11]1.Br[c:5]1[cH:4][cH:3][c:2]([OH:1])[cH:13][cH:12]1>>[OH:1][c:2]1[cH:3][cH:4][c:5](-[c:6]2[cH:7][cH:8][cH:9][n:10][cH:11]2)[cH:12][cH:13]1
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1cccnc1.Oc1ccc(Br)cc1
Oc1ccc(-c2cccnc2)cc1
null
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl
O1CCOCC1
C-C Coupling
Stille reaction_aryl
ce918bbb171f9e7bd99035931c043f0f33f636d165d8c0e73629d8717d6c595a
db27eeefac0475c6d74fa10b3167e95a61caaae74e8bbafd45892452c0c3d4d6
c1ccc(-c2cccnc2)cc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].C-C-C-[CH2]-[Sn](-[CH2]-C-C-C)(-[CH2]-C-C-C)-[c;H0;D3;+0:6]1:[c:7]:[#7;a:8]:[c:9]:[c:10]:[c:11]:1>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6]1:[c:7]:[#7;a:8]:[c:9]:[c:10]:[c:11]:1):[c:4]:[c:5]
60
[{"value": 60.0, "product": "N1=CC(=CC=C1)C1=CC=C(C=C1)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
26.8 g of 4-bromophenol was taken under protective gas in 1000 ml of dioxane, mixed with 90 g 3-tributylstannylpyridine [preparation according to litt.: Org. Magn. Resonance, 7 (1975), 610] and 11.1 g of bis-(triphenylphosphine)-palladium(II) chloride and refluxed for 15 hours. After concentration by evaporation in a v...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Tin
null
c1ccncc1.c1ccccc1
c1ccccc1.c1ccncc1
c1ccccc1.c1ccncc1
HBr.Sn
Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.O1CCOCC1
null
null
CCC[CH2][Sn]([CH2]CCC)([CH2]CCC)[c]1cccnc1.Oc1ccc(Br)cc1>Cl[Pd]([P](C1=CC=CC=C1)(C2=CC=CC=C2)C3=CC=CC=C3)([P](C4=CC=CC=C4)(C5=CC=CC=C5)C6=CC=CC=C6)Cl.O1CCOCC1>Oc1ccc(-c2cccnc2)cc1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-4aeb686c490442b0b6a3ee76700a4b23
CN.COC(=O)c1ccnc(NCCCN2CCN(c3cccc(Cl)c3)CC2)n1>>CNC(=O)c1ccnc(NCCCN2CCN(c3cccc(Cl)c3)CC2)n1
Cl.ClC=1C=C(C=CC1)N1CCN(CC1)CCCNC1=NC=CC(=N1)C(=O)OC.CO.CN>>Cl.ClC=1C=C(C=CC1)N1CCN(CC1)CCCNC1=NC=CC(=N1)C(=O)NC
[CH3:1][NH2:2].CO[C:3](=[O:4])[c:5]1[cH:6][cH:7][n:8][c:9]([NH:10][CH2:11][CH2:12][CH2:13][N:14]2[CH2:15][CH2:16][N:17]([c:18]3[cH:19][cH:20][cH:21][c:22]([Cl:23])[cH:24]3)[CH2:25][CH2:26]2)[n:27]1>>[CH3:1][NH:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][n:8][c:9]([NH:10][CH2:11][CH2:12][CH2:13][N:14]2[CH2:15][CH2:16][N:17]([c:18...
CN.COC(=O)c1ccnc(NCCCN2CCN(c3cccc(Cl)c3)CC2)n1
CNC(=O)c1ccnc(NCCCN2CCN(c3cccc(Cl)c3)CC2)n1
null
null
CC(C)O
Acylation
Aminolysis of esters
04c54ce22aa9bc0cea0de3d900446bcab51cf02bebeb606fa788a47dcd0e37ff
4335147c9ad02004b7c12428d7eac0b2e7e0e2017adc471d01c387239de8017d
c1ccc(N2CCN(CCCNc3ncccn3)CC2)cc1
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:[c:8]:1.[C;D1;H3:9]-[NH2;D1;+0:10]>>[C;D1;H3:9]-[NH;D2;+0:10]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:[c:8]:1
null
[]
null
null
null
null
4.5 g (11.5 mmols) of methyl 2-[[3-[4-(3-chlorophenyl)piperazin-1-yl]propyl]amino]pyrimidine-4-carboxylate and 200 ml of methanol are introduced into a 0.5 l, round bottomed flask and then the solution is saturated with gaseous methylamine. The reaction mixture is stirred at room temperature while saturating several ti...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine
Secondary amide
null
null
c1cncnc1.C1C[NH]CC[NH]1.c1ccccc1
HO-
CC(C)O
null
null
CN.COC(=O)c1ccnc(NCCCN2CCN(c3cccc(Cl)c3)CC2)n1>CC(C)O>CNC(=O)c1ccnc(NCCCN2CCN(c3cccc(Cl)c3)CC2)n1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-682b7c7c9d9d4c65b29faad31f704d69
COC(=O)c1ccnc(NCCCN2CCN(c3cc(Cl)ccc3OC)CC2)n1.NCCNc1nc(=O)cc[nH]1>>COc1ccc(Cl)cc1N1CCN(CCCNc2nccc(C(=O)NCCNc3nc(=O)cc[nH]3)n2)CC1
ClC=1C=CC(=C(C1)N1CCN(CC1)CCCNC1=NC=CC(=N1)C(=O)OC)OC.NCCNC=1NC=CC(N1)=O>>ClC=1C=CC(=C(C1)N1CCN(CC1)CCCNC1=NC=CC(=N1)C(=O)NCCNC=1NC=CC(N1)=O)OC
CO[C:23]([c:22]1[cH:21][cH:20][n:19][c:18]([NH:17][CH2:16][CH2:15][CH2:14][N:13]2[CH2:12][CH2:11][N:10]([c:9]3[c:3]([O:2][CH3:1])[cH:4][cH:5][c:6]([Cl:7])[cH:8]3)[CH2:38][CH2:37]2)[n:36]1)=[O:24].[NH2:25][CH2:26][CH2:27][NH:28][c:29]1[n:30][c:31](=[O:32])[cH:33][cH:34][nH:35]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([Cl:7...
COC(=O)c1ccnc(NCCCN2CCN(c3cc(Cl)ccc3OC)CC2)n1.NCCNc1nc(=O)cc[nH]1
COc1ccc(Cl)cc1N1CCN(CCCNc2nccc(C(=O)NCCNc3nc(=O)cc[nH]3)n2)CC1
null
null
C(CCC)O
Acylation
Aminolysis of esters
04c54ce22aa9bc0cea0de3d900446bcab51cf02bebeb606fa788a47dcd0e37ff
4335147c9ad02004b7c12428d7eac0b2e7e0e2017adc471d01c387239de8017d
O=C(NCCNc1nc(=O)cc[nH]1)c1ccnc(NCCCN2CCN(c3ccccc3)CC2)n1
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:[c:8]:1.[C:9]-[C:10]-[NH2;D1;+0:11]>>[C:9]-[C:10]-[NH;D2;+0:11]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:[c:8]:1
null
[]
null
null
null
null
1.89 g of (4.5 mmols) of methyl 2-[[3-[4-(5-chloro-2-methoxyphenyl)piperazin-1-yl]propyl]amino]-pyrimidine-4-carboxylate and 0.77 g (5 mmols) of 2-[(2-aminoethyl)amino]pyrimidin-4(1H)-one in 5 ml of n-butanol are introduced into a 25 ml, round bottomed flask. The mixture is heated at the reflux temperature of the solve...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine
Secondary amide
null
null
c1ccccc1.C1C[NH]CC[NH]1.c1cncnc1.c1ccncn1
HO-
C(CCC)O
null
null
COC(=O)c1ccnc(NCCCN2CCN(c3cc(Cl)ccc3OC)CC2)n1.NCCNc1nc(=O)cc[nH]1>C(CCC)O>COc1ccc(Cl)cc1N1CCN(CCCNc2nccc(C(=O)NCCNc3nc(=O)cc[nH]3)n2)CC1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-61c8410b006347f6bdbec94f311bc8c4
COC(=O)c1ccnc(NCCN2CCN(c3cc(Cl)ccc3OC)CC2)n1.NCCCNc1nc(=O)cc[nH]1>>COc1ccc(Cl)cc1N1CCN(CCNc2nccc(C(=O)NCCCNc3nc(=O)cc[nH]3)n2)CC1
ClC=1C=CC(=C(C1)N1CCN(CC1)CCNC1=NC=CC(=N1)C(=O)OC)OC.NCCCNC=1NC=CC(N1)=O>>ClC=1C=CC(=C(C1)N1CCN(CC1)CCNC1=NC=CC(=N1)C(=O)NCCCNC=1NC=CC(N1)=O)OC
CO[C:22]([c:21]1[cH:20][cH:19][n:18][c:17]([NH:16][CH2:15][CH2:14][N:13]2[CH2:12][CH2:11][N:10]([c:9]3[c:3]([O:2][CH3:1])[cH:4][cH:5][c:6]([Cl:7])[cH:8]3)[CH2:38][CH2:37]2)[n:36]1)=[O:23].[NH2:24][CH2:25][CH2:26][CH2:27][NH:28][c:29]1[n:30][c:31](=[O:32])[cH:33][cH:34][nH:35]1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([Cl:7...
COC(=O)c1ccnc(NCCN2CCN(c3cc(Cl)ccc3OC)CC2)n1.NCCCNc1nc(=O)cc[nH]1
COc1ccc(Cl)cc1N1CCN(CCNc2nccc(C(=O)NCCCNc3nc(=O)cc[nH]3)n2)CC1
null
null
C(CCC)O
Acylation
Aminolysis of esters
04c54ce22aa9bc0cea0de3d900446bcab51cf02bebeb606fa788a47dcd0e37ff
4335147c9ad02004b7c12428d7eac0b2e7e0e2017adc471d01c387239de8017d
O=C(NCCCNc1nc(=O)cc[nH]1)c1ccnc(NCCN2CCN(c3ccccc3)CC2)n1
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:[c:8]:1.[C:9]-[C:10]-[NH2;D1;+0:11]>>[C:9]-[C:10]-[NH;D2;+0:11]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[#7;a:4]:[c:5]:[#7;a:6]:[c:7]:[c:8]:1
null
[]
null
null
null
null
3.0 g (7.4 mmols) of methyl 2-[[2-[4-(5-chloro-2-methoxyphenyl)piperazin- 1-yl]ethyl]amino]-pyrimidine-4-carboxylate and 1.5 g (8.9 mmols) of 2-[(3-aminopropyl)amino]pyrimidin-4(1H)-one in 20 ml of n-butanol are introduced into a 100 ml, round bottomed flask. The mixture is heated at the reflux temperature of the solve...
10.6084/m9.figshare.5104873.v1
null
Ester.Primary amine
Secondary amide
null
null
c1ccccc1.C1C[NH]CC[NH]1.c1cncnc1.c1ccncn1
HO-
C(CCC)O
null
null
COC(=O)c1ccnc(NCCN2CCN(c3cc(Cl)ccc3OC)CC2)n1.NCCCNc1nc(=O)cc[nH]1>C(CCC)O>COc1ccc(Cl)cc1N1CCN(CCNc2nccc(C(=O)NCCCNc3nc(=O)cc[nH]3)n2)CC1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-d740cb40c09548b39dbf951d10f89106
COc1ccc(Cl)cc1N1CCN(CCNc2nccc(C(=O)N3CCC(N)CC3)n2)CC1.CSc1nc(=O)cc[nH]1>>COc1ccc(Cl)cc1N1CCN(CCNc2nccc(C(=O)N3CCC(Nc4nc(=O)cc[nH]4)CC3)n2)CC1
ClC=1C=CC(=C(C1)N1CCN(CC1)CCNC1=NC=CC(=N1)C(=O)N1CCC(CC1)N)OC.CSC=1NC=CC(N1)=O>>ClC=1C=CC(=C(C1)N1CCN(CC1)CCNC1=NC=CC(=N1)C(=O)N1CCC(CC1)NC=1NC=CC(N1)=O)OC
[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([Cl:7])[cH:8][c:9]1[N:10]1[CH2:11][CH2:12][N:13]([CH2:14][CH2:15][NH:16][c:17]2[n:18][cH:19][cH:20][c:21]([C:22](=[O:23])[N:24]3[CH2:25][CH2:26][CH:27]([NH2:28])[CH2:36][CH2:37]3)[n:38]2)[CH2:39][CH2:40]1.CS[c:29]1[n:30][c:31](=[O:32])[cH:33][cH:34][nH:35]1>>[CH3:1][O:2][c:3]1[cH:4][...
COc1ccc(Cl)cc1N1CCN(CCNc2nccc(C(=O)N3CCC(N)CC3)n2)CC1.CSc1nc(=O)cc[nH]1
COc1ccc(Cl)cc1N1CCN(CCNc2nccc(C(=O)N3CCC(Nc4nc(=O)cc[nH]4)CC3)n2)CC1
null
null
C1(=CC(=CC=C1)C)C
Heteroatom Alkylation and Arylation
OtherReaction
5f2ea2586cfa2f11d765b05bd73f877d3eba93e8a380c059f41d4627fde15d79
88e0224d19b2dce8f9987d52554afb32090d36ff7ee19e89dc5bf66d30974ec4
O=C(c1ccnc(NCCN2CCN(c3ccccc3)CC2)n1)N1CCC(Nc2nc(=O)cc[nH]2)CC1
C-S-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[#7;a:4]:[c:5].[C:6]-[C:7](-[NH2;D1;+0:8])-[C:9]>>[C:6]-[C:7](-[NH;D2;+0:8]-[c;H0;D3;+0:1](:[#7;a:2]:[c:3]):[#7;a:4]:[c:5])-[C:9]
55.9
[{"value": 55.9, "product": "ClC=1C=CC(=C(C1)N1CCN(CC1)CCNC1=NC=CC(=N1)C(=O)N1CCC(CC1)NC=1NC=CC(N1)=O)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
2.3 g (4.9 mmol) of 1-[2-[[2-[4-(5-chloro-2-methoxyphenyl)piperazin-1-yl]ethyl]amino]pyrimidin-4-ylcarbonyl]piperidin-4-amine, and 0.9 g (6.3 mmols) of 2-methylthiopyrimidin-4(1H)-one in solution in 40 ml of m-xylene are introduced into a 0.5 l, round bottomed flask and the mixture is heated at reflux of the m-xylene f...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Monosulfide
Secondary amine
c1ccncn1
c1ccncn1
c1ccccc1.C1C[NH]CC[NH]1.c1cncnc1.C1CC[NH]CC1.c1ccncn1
Other
C1(=CC(=CC=C1)C)C
null
null
COc1ccc(Cl)cc1N1CCN(CCNc2nccc(C(=O)N3CCC(N)CC3)n2)CC1.CSc1nc(=O)cc[nH]1>C1(=CC(=CC=C1)C)C>COc1ccc(Cl)cc1N1CCN(CCNc2nccc(C(=O)N3CCC(Nc4nc(=O)cc[nH]4)CC3)n2)CC1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-29b1539b5e8e4303be8267bfa4999d0d
CCOC(=O)C(=O)OCC.COc1ccc(Br)c(C(C)C(=O)[O-])c1>>CCOC(=O)C(=O)C(Cc1cc(OC)ccc1Br)C(=O)OCC
O.CC(C)([O-])C.[K+].BrC1=C(C=C(C=C1)OC)C(C(=O)[O-])C.C(C(=O)OCC)(=O)OCC.CCOCC.CCOCC>>O=C(C(=O)OCC)C(CC1=C(C=CC(=C1)OC)Br)C(=O)OCC
[CH3:1][CH2:2][O:3][C:4](=[O:5])[C:6](=[O:7])[O:21][CH2:22][CH3:23].[O-][C:19]([CH:8]([CH3:9])[c:10]1[cH:11][c:12]([O:13][CH3:14])[cH:15][cH:16][c:17]1[Br:18])=[O:20]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[C:6](=[O:7])[CH:8]([CH2:9][c:10]1[cH:11][c:12]([O:13][CH3:14])[cH:15][cH:16][c:17]1[Br:18])[C:19](=[O:20])[O:21][CH2:22...
CCOC(=O)C(=O)OCC.COc1ccc(Br)c(C(C)C(=O)[O-])c1
CCOC(=O)C(=O)C(Cc1cc(OC)ccc1Br)C(=O)OCC
null
null
null
C-C Coupling
OtherReaction
a5d192f9fabd52ac26c08069b9ccd9bdf3bf887257f96bffa9fa72c098f21d83
d4410d30228c25b48f58ac92bab260611786b9e684966602ec75966220b57fba
c1ccccc1
[Br;D1;H0:1]-[c:2](:[c:3]):[c;H0;D3;+0:4](-[CH;D3;+0:5](-[CH3;D1;+0:6])-[C;H0;D3;+0:7](-[O-])=[O;D1;H0:8]):[c:9]:[c:10].[C:11]-[#8:12]-[C:13](=[O;D1;H0:14])-[C;H0;D3;+0:15](=[O;D1;H0:16])-[O;H0;D2;+0:17]-[C:18]-[C;D1;H3:19]>>[Br;D1;H0:1]-[c:2](:[c:3]):[c;H0;D3;+0:4](-[CH2;D2;+0:6]-[CH;D3;+0:5](-[C;H0;D3;+0:7](=[O;D1;H0...
90
[{"value": 90.0, "product": "O=C(C(=O)OCC)C(CC1=C(C=CC(=C1)OC)Br)C(=O)OCC", "details": "PERCENTYIELD", "is_desired": false}]
0
CELSIUS
null
null
Potassium t-butoxide (6.72 g) was suspended in 30 ml of anhydrous ether and cooled to 0° C. A solution of 14.35 g of ethyl 3-(2-bromo-5-methoxyphenyl-propionate and 10.95 g diethyl oxalate in 10 ml ether was added dropwise over 15 min. After 2 at 25° C., the reaction was poured into 100 ml H2O and the aqueous layer was...
10.6084/m9.figshare.5104873.v1
null
Ester.Ester
Ketone.Ester.Ester
c1ccccc1
c1ccccc1
c1ccccc1
HO-
null
0
null
CCOC(=O)C(=O)OCC.COc1ccc(Br)c(C(C)C(=O)[O-])c1>>CCOC(=O)C(=O)C(Cc1cc(OC)ccc1Br)C(=O)OCC
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-09ecf8fbcf7143b4b4b1bb485c9c30d9
CCOC(=O)C1=C(C(=O)OCC)c2c(OC)ccc(Br)c2C1>>CCOC(=O)C1Cc2cccc(OC)c2C1C(=O)OCC
BrC=1C=CC(=C2C(=C(CC12)C(=O)OCC)C(=O)OCC)OC>>COC1=C2C(C(CC2=CC=C1)C(=O)OCC)C(=O)OCC
Br[c:9]1[c:8]2[c:15]([c:12]([O:13][CH3:14])[cH:11][cH:10]1)[C:16]([C:17](=[O:18])[O:19][CH2:20][CH3:21])=[C:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[CH2:7]2>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]1[CH2:7][c:8]2[cH:9][cH:10][cH:11][c:12]([O:13][CH3:14])[c:15]2[CH:16]1[C:17](=[O:18])[O:19][CH2:20][CH3:21]
CCOC(=O)C1=C(C(=O)OCC)c2c(OC)ccc(Br)c2C1
CCOC(=O)C1Cc2cccc(OC)c2C1C(=O)OCC
null
[Pd].[O-]S(=O)(=O)[O-].[Ba+2]
C(C)O
Reduction
OtherReaction
00ee50f454e9483f7fd1bf0416428eb028e8c793c0f9d9e39b946a0cad0350d0
3b66793f09edb4afa775171d5142cfc257af0edb413721d00ecd4602c93c6b9e
c1ccc2c(c1)CCC2
Br-[c;H0;D3;+0:1]1:[c:2]:[c:3]:[c:4]:[c:5]2:[c:6]:1-[C:7]-[C;H0;D3;+0:8](-[C:9](=[O;D1;H0:10])-[#8:11]-[C:12])=[C;H0;D3;+0:13]-2-[C:14](=[O;D1;H0:15])-[#8:16]-[C:17]>>[C:17]-[#8:16]-[C:14](=[O;D1;H0:15])-[CH;D3;+0:13]1-[CH;D3;+0:8](-[C:9](=[O;D1;H0:10])-[#8:11]-[C:12])-[C:7]-[c:6]2:[cH;D2;+0:1]:[c:2]:[c:3]:[c:4]:[c:5]:...
96.9
[{"value": 96.9, "product": "COC1=C2C(C(CC2=CC=C1)C(=O)OCC)C(=O)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
The diester from Example 2 (19.39 g) was dissolved in 250 ml ethanol. To the solution was added 5.20 g of 10% Pd/BaSO4 and 7.15 g NaOAc.3H2O. The reaction was hydrogenated at 4 atm pressure. The catalyst was filtered and the solvent evaporated. The product was dissolved in ether, washed with 5% NaHCO3, dried (MgSO4), a...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ester.Ester
Ester.Ester
C1=Cc2ccccc2C1
c1ccc2c(c1)CCC2
c1ccc2c(c1)CCC2
Br-
[Pd].[O-]S(=O)(=O)[O-].[Ba+2].C(C)O
null
null
CCOC(=O)C1=C(C(=O)OCC)c2c(OC)ccc(Br)c2C1>[Pd].[O-]S(=O)(=O)[O-].[Ba+2].C(C)O>CCOC(=O)C1Cc2cccc(OC)c2C1C(=O)OCC
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-7fb126bc875649eb8713b2431fdb30fa
COC1c2ccccc2C2CN(Cc3ccccc3)CC21>>COC1c2ccccc2C2CNCC21
Cl.C(C1=CC=CC=C1)N1CC2C(C1)C(C=1C=CC=CC12)OC>>Cl.COC1C=2C=CC=CC2C2CNCC21
c1ccc(C[N:12]2[CH2:11][CH:10]3[c:9]4[c:4]([cH:5][cH:6][cH:7][cH:8]4)[CH:3]([O:2][CH3:1])[CH:14]3[CH2:13]2)cc1>>[CH3:1][O:2][CH:3]1[c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2[CH:10]2[CH2:11][NH:12][CH2:13][CH:14]12
COC1c2ccccc2C2CN(Cc3ccccc3)CC21
COC1c2ccccc2C2CNCC21
null
[Pd]
CO
Deprotection
Hydrogenolysis of tertiary amines
dd42f97580a8f7f0cafefbd81bcf5a8bcbf7040d74f9339d074d65acb45f1646
1c99dd446c0bf4ae872cd8df8de34955be195747c234e9f3c49f46d1de614f66
c1ccc2c(c1)CC1CNCC21
C(-[N;H0;D3;+0:1]1-[C:2]-[C:3]-[C:4]-[C:5]-1)-c1:c:c:c:c:c:1>>[C:3]1-[C:2]-[NH;D2;+0:1]-[C:5]-[C:4]-1
90.5
[{"value": 90.5, "product": "Cl.COC1C=2C=CC=CC2C2CNCC21", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
The product from Example 5 (4.90 g) was hydrogenated with 2.45 g 20% Pd/C in 200 ml methanol at 3 atm, affording 3.17 g of the desired product, mp: 208°-209° C. NMR (d6DMSO/D2O) δ2.83 (m, 2H), 3.14-3.29 (m, 3H), 3.46 (dd, 1H), 3.55 (dd, 1H), 3.80 (s, 3H), 3.95 (m, 1H), 6.85 (d, 2H), 7.25 (t, 1H). Conditions: See reacti...
10.6084/m9.figshare.5104873.v1
null
Tertiary amine
Secondary amine
c1ccccc1.c1ccc2c(c1)CC1C[NH]CC21
c1ccc2c(c1)CC1CNCC21
c1ccc2c(c1)CC1CNCC21
Other
[Pd].CO
null
null
COC1c2ccccc2C2CN(Cc3ccccc3)CC21>[Pd].CO>COC1c2ccccc2C2CNCC21
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-fb02e62a59a44836a806f3943ed12dcc
BrB(Br)Br.CCCN1CC2c3ccccc3C(OC)C2C1>>Br.CCCN1CC2c3ccccc3C(O)C2C1
Cl.COC1C=2C=CC=CC2C2CN(CC21)CCC.B(Br)(Br)Br>>Br.OC1C=2C=CC=CC2C2CN(CC21)CCC
BrB(Br)[Br:1].C[O:15][CH:14]1[c:13]2[c:8]([cH:9][cH:10][cH:11][cH:12]2)[CH:7]2[CH2:6][N:5]([CH2:4][CH2:3][CH3:2])[CH2:17][CH:16]21>>[BrH:1].[CH3:2][CH2:3][CH2:4][N:5]1[CH2:6][CH:7]2[c:8]3[cH:9][cH:10][cH:11][cH:12][c:13]3[CH:14]([OH:15])[CH:16]2[CH2:17]1
BrB(Br)Br.CCCN1CC2c3ccccc3C(OC)C2C1
Br.CCCN1CC2c3ccccc3C(O)C2C1
null
null
C(Cl)Cl
Miscellaneous
OtherReaction
033263114fa374bfee35f27920670e8f6275414faa199071efed4247f43e41f8
816a42e4e92b4becc10e09218671f2e2a7942c9348b22e40d965e6444e589265
c1ccc2c(c1)CC1CNCC21
Br-B(-Br)-[Br;H0;D1;+0:1].C-[O;H0;D2;+0:2]-[C:3](-[C:4])-[c:5]>>[BrH;D0;+0:1].[C:4]-[C:3](-[OH;D1;+0:2])-[c:5]
null
[]
-78
CELSIUS
null
null
The product from Example 9 (0.490 g) was dissolved in 25 ml methylene chloride and cooled to -78° C. To the reaction was added 0.69 ml BBr3. The reaction was warmed to 0° C. for 4 h and then cooled to -78° C. The reaction was quenched by the addition of 5 ml methanol and the solvent was evaporated. The resulting solid ...
10.6084/m9.figshare.5104873.v1
null
Ether
Secondary alcohol
null
null
c1ccc2c(c1)CC1C[NH]CC21
HBr.B
C(Cl)Cl
-78
null
BrB(Br)Br.CCCN1CC2c3ccccc3C(OC)C2C1>C(Cl)Cl>Br.CCCN1CC2c3ccccc3C(O)C2C1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-b8624136abe04640a5b5ceda72784b10
COC1c2ccccc2C2CN(CC#N)CC21>>COC1c2ccccc2C2CN(CCN)CC21
COC1C=2C=CC=CC2C2CN(CC21)CC#N>>COC1C=2C=CC=CC2C2CN(CC21)CCN
[CH3:1][O:2][CH:3]1[c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2[CH:10]2[CH2:11][N:12]([CH2:13][C:14]#[N:15])[CH2:16][CH:17]12>>[CH3:1][O:2][CH:3]1[c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2[CH:10]2[CH2:11][N:12]([CH2:13][CH2:14][NH2:15])[CH2:16][CH:17]12
COC1c2ccccc2C2CN(CC#N)CC21
COC1c2ccccc2C2CN(CCN)CC21
null
[Rh]
CO.N
Reduction
Reduction of nitrile to amine
65bec2d9f430701d30dc9fcbe1c5418f3dfa174d67be035c50edfc71895dc9c7
e8d1bc928b94bd4f5bf4b23363ce8f88b1ce7d146ba93829e7b8ad8dbe0007a7
c1ccc2c(c1)CC1CNCC21
[#7:1]-[C:2]-[C;H0;D2;+0:3]#[N;H0;D1;+0:4]>>[#7:1]-[C:2]-[CH2;D2;+0:3]-[NH2;D1;+0:4]
95.3
[{"value": 95.3, "product": "COC1C=2C=CC=CC2C2CN(CC21)CCN", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
4
HOUR
The product from Example 16 (1.00 g) was dissolved in 90 ml methanol and 10 ml anhydrous ammonia. 0.100 g 5% Rh/Al2O3 was added and the reaction was hydrogenated at 4 atm for 4 h. The reaction was filtered and the solvent removed to yield 0.97 g of the desired product as a colorless oil. NMR (CDCl3) δ2.20-2.61 (m, 3H),...
10.6084/m9.figshare.5104873.v1
null
Nitrile
Primary amine
null
null
c1ccc2c(c1)CC1C[NH]CC21
null
[Rh].CO.N
null
4
COC1c2ccccc2C2CN(CC#N)CC21>[Rh].CO.N>COC1c2ccccc2C2CN(CCN)CC21
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-f54e63fe817945f5aca1b6509ef67a57
COC1c2ccccc2C2CN(CCN)CC21.O=C(Cl)c1ccc(F)cc1>>COC1c2ccccc2C2CN(CCNC(=O)c3ccc(F)cc3)CC21.Cl
COC1C=2C=CC=CC2C2CN(CC21)CCN.FC1=CC=C(C(=O)Cl)C=C1>>Cl.COC1C=2C=CC=CC2C2CN(CC21)CCNC(C2=CC=C(C=C2)F)=O
[CH3:1][O:2][CH:3]1[c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2[CH:10]2[CH2:11][N:12]([CH2:13][CH2:14][NH2:15])[CH2:25][CH:26]12.[C:16](=[O:17])([c:18]1[cH:19][cH:20][c:21]([F:22])[cH:23][cH:24]1)[Cl:27]>>[CH3:1][O:2][CH:3]1[c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2[CH:10]2[CH2:11][N:12]([CH2:13][CH2:14][NH:15][C:16](=[O:17])[c:18]3...
COC1c2ccccc2C2CN(CCN)CC21.O=C(Cl)c1ccc(F)cc1
COC1c2ccccc2C2CN(CCNC(=O)c3ccc(F)cc3)CC21.Cl
null
null
C(Cl)Cl.C(C)N(CC)CC
Acylation
Acylation of Nitrogen Nucleophiles by Acyl/Thioacyl/Carbamoyl Halides and Analogs_OS
38143a4d536201990008fd6f2c68e6571a341d1c367481869fbbbe36cb038937
0e6ae078978e324f714e184b4f72826d4e3bf2d9ab22d6e9f73740af687be16f
O=C(NCCN1CC2Cc3ccccc3C2C1)c1ccccc1
[C:1]-[C:2]-[NH2;D1;+0:3].[Cl;H0;D1;+0:4]-[C;H0;D3;+0:5](=[O;D1;H0:6])-[c:7](:[c:8]):[c:9]>>[C:1]-[C:2]-[NH;D2;+0:3]-[C;H0;D3;+0:5](=[O;D1;H0:6])-[c:7](:[c:8]):[c:9].[ClH;D0;+0:4]
null
[]
-20
CELSIUS
30
MINUTE
The product from Example 17 (0.95 g) was dissolved in 50 ml methylene chloride and 1.5 ml triethyl amine. The solution was cooled to -20° C. and 0.59 ml p-fluorobenzoyl chloride was added. After 30 min, the reaction was quenched in 5% NaHCO3 and extracted with ethyl acetate. The organic extracts were dried (Na2SO4), ev...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary amine
Secondary amide
null
null
c1ccc2c(c1)CC1C[NH]CC21.c1ccccc1
null
C(Cl)Cl.C(C)N(CC)CC
-20
0.5
COC1c2ccccc2C2CN(CCN)CC21.O=C(Cl)c1ccc(F)cc1>C(Cl)Cl.C(C)N(CC)CC>COC1c2ccccc2C2CN(CCNC(=O)c3ccc(F)cc3)CC21.Cl
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-0c78cd059b394bef950f6b265b6865dc
CCOC(OCC)OCC.COc1ccc(Br)c2c1C(=O)CC2>>CCOC(OCC)C1Cc2c(Br)ccc(OC)c2C1=O
C(C)(C)N(CC)C(C)C.C(OCC)(OCC)OCC.BrC1=C2CCC(C2=C(C=C1)OC)=O.B(F)(F)F.CCOCC>>C(C)OC(C1C(C2=C(C=CC(=C2C1)Br)OC)=O)OCC
CCO[CH:4]([O:3][CH2:2][CH3:1])[O:5][CH2:6][CH3:7].[CH2:8]1[CH2:9][c:10]2[c:11]([Br:12])[cH:13][cH:14][c:15]([O:16][CH3:17])[c:18]2[C:19]1=[O:20]>>[CH3:1][CH2:2][O:3][CH:4]([O:5][CH2:6][CH3:7])[CH:8]1[CH2:9][c:10]2[c:11]([Br:12])[cH:13][cH:14][c:15]([O:16][CH3:17])[c:18]2[C:19]1=[O:20]
CCOC(OCC)OCC.COc1ccc(Br)c2c1C(=O)CC2
CCOC(OCC)C1Cc2c(Br)ccc(OC)c2C1=O
null
null
C(Cl)Cl
C-C Coupling
OtherReaction
0ccb5acbe1cc0192cb1d36afc7997fa48bf65148c2d46ad3b88a4f6cb2d2f99e
155bcdfe4c4a838582eb097f30902e58c733d6d3e0c4634faa32630a07995baa
O=C1CCc2ccccc21
C-C-O-[CH;D3;+0:1](-[#8:2]-[C:3])-[#8:4]-[C:5].[O;D1;H0:6]=[C:7]1-[CH2;D2;+0:8]-[C:9]-[c:10]:[c:11]-1>>[C:3]-[#8:2]-[CH;D3;+0:1](-[#8:4]-[C:5])-[CH;D3;+0:8]1-[C:9]-[c:10]:[c:11]-[C:7]-1=[O;D1;H0:6]
null
[]
0
CELSIUS
null
null
Triethyl orthoformate (16.5 ml) was cooled to -30° C. and 15.0 ml BF3.Et2O in 50 ml methylene chloride was added. The reaction was warmed to 0° C. for 15 min, and then cooled to -78° C. To the reaction was added 12.05 g of the product from Example 34 in 50 ml methylene chloride, followed by dropwise addition of 19.4 ml...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ether.Ether.Ether
Ketone.Ether.Ether
c1ccc2c(c1)CCC2
c1ccc2c(c1)CCC2
c1ccc2c(c1)CCC2
HO-
C(Cl)Cl
0
null
CCOC(OCC)OCC.COc1ccc(Br)c2c1C(=O)CC2>C(Cl)Cl>CCOC(OCC)C1Cc2c(Br)ccc(OC)c2C1=O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-75841078706c471fb11a460ffbd5dc91
COc1cccc2c1[C@H]1CCN(Cc3ccccc3)C[C@H]1C2>>COc1cccc2c1[C@H]1CCNC[C@H]1C2
Cl.C(C1=CC=CC=C1)N1C[C@@H]2[C@H](CC1)C=1C(=CC=CC1C2)OC>>Cl.COC1=CC=CC=2C[C@@H]3CNCC[C@@H]3C12
c1ccc(C[N:12]2[CH2:11][CH2:10][C@@H:9]3[c:8]4[c:3]([O:2][CH3:1])[cH:4][cH:5][cH:6][c:7]4[CH2:15][C@@H:14]3[CH2:13]2)cc1>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7]2[c:8]1[C@H:9]1[CH2:10][CH2:11][NH:12][CH2:13][C@H:14]1[CH2:15]2
COc1cccc2c1[C@H]1CCN(Cc3ccccc3)C[C@H]1C2
COc1cccc2c1[C@H]1CCNC[C@H]1C2
null
[Pd]
CO
Deprotection
Hydrogenolysis of tertiary amines
3b656f8cdadf0ccb010defa73ceaa399d59e9f35c9cde9dd97ae13bfab1c0834
1c99dd446c0bf4ae872cd8df8de34955be195747c234e9f3c49f46d1de614f66
c1ccc2c(c1)C[C@@H]1CNCC[C@H]21
[C:1]-[C:2]-[N;H0;D3;+0:3](-C-c1:c:c:c:c:c:1)-[C:4]-[C:5]>>[C:1]-[C:2]-[NH;D2;+0:3]-[C:4]-[C:5]
82.6
[{"value": 82.6, "product": "Cl.COC1=CC=CC=2C[C@@H]3CNCC[C@@H]3C12", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
The product from Example 41 (1.80 g) was combined with 0.90 g 20% Pd/C in 100 ml methanol and evaporated to yield 1.08 g of the desired product as a white solid, mp: 140°-3° C. NMR (d6DMSO) δ 1.70 (m, 1H), 2.02 (m, 1H), 2.60 (m, 1H), 2.78-3.30 (m, 7H), 3.77 (s, 3H), 6.80 (d, 1H), 6.84 (d, 1H), 7.15 (t, 1H). Conditions:...
10.6084/m9.figshare.5104873.v1
null
Tertiary amine
Secondary amine
c1ccccc1.c1ccc2c(c1)C[C@@H]1C[NH]CC[C@H]21
c1ccc2c(c1)C[C@@H]1CNCC[C@H]21
c1ccc2c(c1)C[C@@H]1CNCC[C@H]21
Other
[Pd].CO
null
null
COc1cccc2c1[C@H]1CCN(Cc3ccccc3)C[C@H]1C2>[Pd].CO>COc1cccc2c1[C@H]1CCNC[C@H]1C2
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-cc146a0b13854115a3294a70fa64f354
COc1ccc(Br)c2c1C(C#N)C(C#N)CC2>>COc1cccc2c1C(C#N)C(C#N)CC2
BrC1=C2CCC(C(C2=C(C=C1)OC)C#N)C#N.CC(=O)[O-].[Na+]>>COC=1C=CC=C2CCC(C(C12)C#N)C#N
Br[c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[c:8]2[c:7]1[CH2:16][CH2:15][CH:12]([C:13]#[N:14])[CH:9]2[C:10]#[N:11]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][cH:6][c:7]2[c:8]1[CH:9]([C:10]#[N:11])[CH:12]([C:13]#[N:14])[CH2:15][CH2:16]2
COc1ccc(Br)c2c1C(C#N)C(C#N)CC2
COc1cccc2c1C(C#N)C(C#N)CC2
null
[Pd].[O-]S(=O)(=O)[O-].[Ba+2]
CO
Functional Group Interconversion
Aromatic dehalogenation
94addc37b1234c3916ac52b9db2a134e35734d066e92c9df0d41a10d4be2c2b1
56de34d4a44cb25d9380269ee5e138b0f24b40a3a0db22c5508049dc775a861f
c1ccc2c(c1)CCCC2
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](:[c:5])-[C:6]>>[C:6]-[c:4](:[c:5]):[cH;D2;+0:1]:[c:2]:[c:3]
85.1
[{"value": 85.1, "product": "COC=1C=CC=C2CCC(C(C12)C#N)C#N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
The product from Example 53 (2.90 g) was treated with 3.0 g 10% Pd/BaSO4 and 1.36 g NaOAc in 250 ml methanol and hydrogenated at 4 atm for 4 h. The reaction was filtered and evaporated; and the product was dissolved in ethyl acetate, washed with 5% NaHCO3, dried (MgSO4), and evaporated to yield 1.80 g of the desired pr...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2
c1ccc2c(c1)CCCC2
Br-
[Pd].[O-]S(=O)(=O)[O-].[Ba+2].CO
null
null
COc1ccc(Br)c2c1C(C#N)C(C#N)CC2>[Pd].[O-]S(=O)(=O)[O-].[Ba+2].CO>COc1cccc2c1C(C#N)C(C#N)CC2
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-623055db120040d483ebba9a6496e49a
CCOC(=O)C(=O)OCC.CCOC(=O)CCCc1cc(OC)ccc1Br>>CCOC(=O)C(=O)C(CCc1cc(OC)ccc1Br)C(=O)OCC
O.CC(C)([O-])C.[K+].C(C)OC(CCCC1=C(C=CC(=C1)OC)Br)=O.C(C(=O)OCC)(=O)OCC>>C(C)OC(C(C(CCC1=C(C=CC(=C1)OC)Br)C(=O)OCC)=O)=O
CCO[C:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])=[O:7].[CH2:8]([CH2:9][CH2:10][c:11]1[cH:12][c:13]([O:14][CH3:15])[cH:16][cH:17][c:18]1[Br:19])[C:20](=[O:21])[O:22][CH2:23][CH3:24]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[C:6](=[O:7])[CH:8]([CH2:9][CH2:10][c:11]1[cH:12][c:13]([O:14][CH3:15])[cH:16][cH:17][c:18]1[Br:19])[C:20](=[O:2...
CCOC(=O)C(=O)OCC.CCOC(=O)CCCc1cc(OC)ccc1Br
CCOC(=O)C(=O)C(CCc1cc(OC)ccc1Br)C(=O)OCC
null
null
CCOCC
C-C Coupling
OtherReaction
831b39d9ccf68cb6d272eab2c65f66125e8f825272f7523cabe1d45c78ab2fbb
d0be73e10992279cb1102524f458cbe914ec5b996a4c52f764855ef41c8e23eb
c1ccccc1
C-C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](=[O;D1;H0:4])-[#8:5]-[C:6].[C:7]-[C:8]-[CH2;D2;+0:9]-[C:10](=[O;D1;H0:11])-[#8:12]-[C:13]>>[C:7]-[C:8]-[CH;D3;+0:9](-[C:10](=[O;D1;H0:11])-[#8:12]-[C:13])-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](=[O;D1;H0:4])-[#8:5]-[C:6]
89
[{"value": 89.0, "product": "C(C)OC(C(C(CCC1=C(C=CC(=C1)OC)Br)C(=O)OCC)=O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 88.8, "product": "C(C)OC(C(C(CCC1=C(C=CC(=C1)OC)Br)C(=O)OCC)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
2
HOUR
Potassium t-butoxide (26.94 g) was suspended in 130 ml of anhydrous ether and cooled to 0° C. A solution of 60.24 g ethyl -4-(2-bromo-5-methoxy phenyl)butyrate and 43.84 g diethyl oxalate in 60 ml ether was added dropwise over 20 min. After 2 h at 25° C., the reaction was poured into 400 ml H2O and the aqueous layer wa...
10.6084/m9.figshare.5104873.v1
null
Ester.Ester.Ester
Ketone
null
null
c1ccccc1
HO-
CCOCC
0
2
CCOC(=O)C(=O)OCC.CCOC(=O)CCCc1cc(OC)ccc1Br>CCOCC>CCOC(=O)C(=O)C(CCc1cc(OC)ccc1Br)C(=O)OCC
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-1b12255dade444fbb86d1602f50259b7
CN(C)C=O.COC(=O)[C@H](Cc1ccc(O)cc1)NC(=O)OC(C)(C)C>>COCCOCc1cc(O)ccc1C[C@@H](CO)NC(=O)OC(C)(C)C
COC([C@@H](NC(=O)OC(C)(C)C)CC1=CC=C(C=C1)O)=O.[H-].[Na+].[Cl-].[Li+].[BH4-].[Na+].CN(C=O)C>>C(C)(C)(C)OC(=O)N[C@@H](CC1=C(C=C(C=C1)O)COCCOC)CO
N([CH3:3])([CH3:4])[CH:6]=[O:5].[CH3:1][O:2][C:16]([C@H:15]([CH2:14][c:13]1[cH:7][cH:8][c:9]([OH:10])[cH:11][cH:12]1)[NH:18][C:19](=[O:20])[O:21][C:22]([CH3:23])([CH3:24])[CH3:25])=[O:17]>>[CH3:1][O:2][CH2:3][CH2:4][O:5][CH2:6][c:7]1[cH:8][c:9]([OH:10])[cH:11][cH:12][c:13]1[CH2:14][C@@H:15]([CH2:16][OH:17])[NH:18][C:19...
CN(C)C=O.COC(=O)[C@H](Cc1ccc(O)cc1)NC(=O)OC(C)(C)C
COCCOCc1cc(O)ccc1C[C@@H](CO)NC(=O)OC(C)(C)C
null
null
C(C)O.O1CCCC1
Heteroatom Alkylation and Arylation
OtherReaction
00d452f033d2acdebf3ac4c04c76e70023edc8026121ba0d8470b5f4d221eced
4ce9596af059d87d7f691a50ccc0b4745b9b3eeabaf308152f422c9f89fd584c
c1ccccc1
[C;D1;H3:1]-[O;H0;D2;+0:2]-[C;H0;D3;+0:3](=[O;H0;D1;+0:4])-[C:5](-[#7:6]-[C:7](=[O;D1;H0:8])-[#8:9]-[C:10](-[C;D1;H3:11])(-[C;D1;H3:12])-[C;D1;H3:13])-[C:14]-[c:15](:[c:16]):[cH;D2;+0:17]:[c:18]:[c:19].[CH3;D1;+0:20]-N(-[CH3;D1;+0:21])-[CH;D2;+0:22]=[O;H0;D1;+0:23]>>[C;D1;H3:1]-[O;H0;D2;+0:2]-[CH2;D2;+0:20]-[CH2;D2;+0:...
null
[]
null
null
null
null
13.39 g of N-t-butoxycarbonyltyrosine methyl ester was dissolved in 65 ml of tetrahydrofuran and 65 ml of dimethylformamide. 1.9 g of 60% sodium hydride was added to the solution under stirring while ice-cooled. After the ice bath was removed, the mixture was stirred at room temperature for 30 minutes and then 5.4 g of...
10.6084/m9.figshare.5104873.v1
null
Ester.Tertiary amide
Ether.Ether.Primary alcohol
c1ccccc1
c1ccccc1
c1ccccc1
Other
C(C)O.O1CCCC1
null
null
CN(C)C=O.COC(=O)[C@H](Cc1ccc(O)cc1)NC(=O)OC(C)(C)C>C(C)O.O1CCCC1>COCCOCc1cc(O)ccc1C[C@@H](CO)NC(=O)OC(C)(C)C
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-e4a23dd9d11840d1854afd3d74c6084e
CCOC(=O)c1c(S(C)=O)sc2ccccc2c1=O>>CCOC(=O)c1c(S)sc2ccccc2c1=O
C(C)OC(=O)C1=C(SC2=C(C1=O)C=CC=C2)S(=O)C.S.[Na]>>C(C)OC(=O)C1=C(SC2=C(C1=O)C=CC=C2)S
C[S:8](=O)[c:7]1[c:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[c:16](=[O:17])[c:15]2[c:10]([s:9]1)[cH:11][cH:12][cH:13][cH:14]2>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[c:7]([SH:8])[s:9][c:10]2[cH:11][cH:12][cH:13][cH:14][c:15]2[c:16]1=[O:17]
CCOC(=O)c1c(S(C)=O)sc2ccccc2c1=O
CCOC(=O)c1c(S)sc2ccccc2c1=O
null
null
O1CCCC1
Miscellaneous
OtherReaction
eef2e1b5ff0f69ab6081f09517432c05434b0ab0589dc0e3684a9e4e2f78d988
b886beeb8fbfa84bb0f92183b9fe913660dce69c18077df92371b7c354b5aef5
O=c1ccsc2ccccc12
C-[S;H0;D3;+0:1](=O)-[c:2](:[#16;a:3]:[c:4]):[c:5]-[C:6](-[#8:7])=[O;D1;H0:8]>>[#8:7]-[C:6](=[O;D1;H0:8])-[c:5]:[c:2](-[SH;D1;+0:1]):[#16;a:3]:[c:4]
23
[{"value": 23.0, "product": "C(C)OC(=O)C1=C(SC2=C(C1=O)C=CC=C2)S", "details": "PERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
To a solution of 100 mg (0.337 mmol) of the compound of Example 18 in 1.8 ml of tetrahydrofuran was added 1N sodium hydrogensulfide (0.697 mmol), and the mixture was stirred for 3 hours. Solvent was distilled off and 87 mg of sodium bicarbonate and 6.5 ml of water were added to the residue, which was washed with dichlo...
10.6084/m9.figshare.5104873.v1
null
Sulfoxide
Aromatic thiol
null
null
c1csc2ccccc2c1
HO-
O1CCCC1
null
3
CCOC(=O)c1c(S(C)=O)sc2ccccc2c1=O>O1CCCC1>CCOC(=O)c1c(S)sc2ccccc2c1=O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-c84f1c46a858498aa1a36a9d1af38093
CI.COc1cc(C=O)c(Br)c(Cl)c1O>>COc1cc(C=O)c(Br)c(Cl)c1OC
BrC1=C(C(=C(C=C1C=O)OC)O)Cl.C1CCC2=NCCCN2CC1.CI.C(C)(C)N(CC)C(C)C.CI>>BrC1=C(C=O)C=C(C(=C1Cl)OC)OC
I[CH3:14].[CH3:1][O:2][c:3]1[cH:4][c:5]([CH:6]=[O:7])[c:8]([Br:9])[c:10]([Cl:11])[c:12]1[OH:13]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([CH:6]=[O:7])[c:8]([Br:9])[c:10]([Cl:11])[c:12]1[O:13][CH3:14]
CI.COc1cc(C=O)c(Br)c(Cl)c1O
COc1cc(C=O)c(Br)c(Cl)c1OC
null
null
C(C)#N
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
b8b041187bac58376aae824630608e7deb49a01db3d652291f8b379c10d4e434
0f0966e3597a58033417ecee71659f4d0c082f95d46b1e52c95541e6e4a59086
c1ccccc1
I-[CH3;D1;+0:1].[OH;D1;+0:2]-[c:3](:[c:4]):[c:5]>>[CH3;D1;+0:1]-[O;H0;D2;+0:2]-[c:3](:[c:4]):[c:5]
71
[{"value": 71.0, "product": "BrC1=C(C=O)C=C(C(=C1Cl)OC)OC", "details": "PERCENTYIELD", "is_desired": false}]
null
null
5
HOUR
Into 50 ml of acetonitrile were suspended 5.39 g (20.3 mmol), of 6-bromo-5-chlorovanillin, and 3.04 ml (20.3 mmol) of 1.8-diazabicyclo[5,4,0]-7-undecene and 2.53 ml (40.6 mmol) of methyl iodide were added dropwise under cooling with ice. After stirred for 5 hours at room temperature, 3.9 ml (22.33 mmol) if diisopropyle...
10.6084/m9.figshare.5104873.v1
null
Aromatic alcohol
Ether
null
null
c1ccccc1
HI
C(C)#N
null
5
CI.COc1cc(C=O)c(Br)c(Cl)c1O>C(C)#N>COc1cc(C=O)c(Br)c(Cl)c1OC
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-93c2e2181a674049914d3893aea5bed6
CCOC(=O)CC(=O)c1cc(F)c(F)c(F)c1F.CI.S=C=S>>CCOC(=O)c1c(SC)sc2c(F)c(F)c(F)cc2c1=O
CI.FC1=C(C(=O)CC(=O)OCC)C=C(C(=C1F)F)F.C(=S)=S.C(C)N(CC)CC>>C(C)OC(=O)C1=C(SC2=C(C1=O)C=C(C(=C2F)F)F)SC
F[c:11]1[c:12]([F:13])[c:14]([F:15])[c:16]([F:17])[cH:18][c:19]1[C:20]([CH2:6][C:4]([O:3][CH2:2][CH3:1])=[O:5])=[O:21].I[CH3:9].[C:7](=[S:8])=[S:10]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[c:6]1[c:7]([S:8][CH3:9])[s:10][c:11]2[c:12]([F:13])[c:14]([F:15])[c:16]([F:17])[cH:18][c:19]2[c:20]1=[O:21]
CCOC(=O)CC(=O)c1cc(F)c(F)c(F)c1F.CI.S=C=S
CCOC(=O)c1c(SC)sc2c(F)c(F)c(F)cc2c1=O
null
null
CS(=O)C
Aromatic Heterocycle Formation
OtherReaction
90930908a1d7a3ae484483ce3381026d7c953f2f3989c0c515d480494eb0dab3
fb7d04511983b89b4e1f5337b203cdb0ea7e85f9161a593cc23135d30f010fdc
O=c1ccsc2ccccc12
F-[c;H0;D3;+0:1](:[c:2](-[F;D1;H0:3]):[c:4]):[c:5](-[C;H0;D3;+0:6](=[O;D1;H0:7])-[CH2;D2;+0:8]-[C:9](=[O;D1;H0:10])-[#8:11]-[C:12]):[c:13].I-[CH3;D1;+0:14].[S;H0;D1;+0:15]=[C;H0;D2;+0:16]=[S;H0;D1;+0:17]>>[C:12]-[#8:11]-[C:9](=[O;D1;H0:10])-[c;H0;D3;+0:8]1:[c;H0;D3;+0:6](=[O;D1;H0:7]):[c:5](:[c:13]):[c;H0;D3;+0:1](:[s;...
74
[{"value": 74.0, "product": "C(C)OC(=O)C1=C(SC2=C(C1=O)C=C(C(=C2F)F)F)SC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 73.8, "product": "C(C)OC(=O)C1=C(SC2=C(C1=O)C=C(C(=C2F)F)F)SC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a solution of 3.00 g (11.4 mmol) of ethyl 2,3,4,5-tetrafluorobenzoylacetate, 870 mg (11.4 mmol) of carbon disulfide and 9 ml of dried dimethyl sulfoxide were added 2.31 g (22.8 mmol) of triethylamine at room temperature, and the mixture was stirred for 1 hour at room temperature. Then, at room temperature, 3.24 g (2...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Ketone.Ester
Ester.Monosulfide
c1ccccc1
c1csc2ccccc2c1
c1csc2ccccc2c1
HF.I-
CS(=O)C
null
1
CCOC(=O)CC(=O)c1cc(F)c(F)c(F)c1F.CI.S=C=S>CS(=O)C>CCOC(=O)c1c(SC)sc2c(F)c(F)c(F)cc2c1=O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-1649d4530bee447eb356e4adaeb56455
CCOC(=O)c1c(SC)sc2c(F)c(F)c(F)cc2c1=O>>CSc1sc2c(F)c(F)c(F)cc2c(=O)c1C(=O)O
C(C)OC(=O)C1=C(SC2=C(C1=O)C=C(C(=C2F)F)F)SC.C(C)(=O)O.S(O)(O)(=O)=O>>C(=O)(O)C1=C(SC2=C(C1=O)C=C(C(=C2F)F)F)SC
CC[O:19][C:17]([c:16]1[c:3]([S:2][CH3:1])[s:4][c:5]2[c:6]([F:7])[c:8]([F:9])[c:10]([F:11])[cH:12][c:13]2[c:14]1=[O:15])=[O:18]>>[CH3:1][S:2][c:3]1[s:4][c:5]2[c:6]([F:7])[c:8]([F:9])[c:10]([F:11])[cH:12][c:13]2[c:14](=[O:15])[c:16]1[C:17](=[O:18])[OH:19]
CCOC(=O)c1c(SC)sc2c(F)c(F)c(F)cc2c1=O
CSc1sc2c(F)c(F)c(F)cc2c(=O)c1C(=O)O
null
null
O
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=c1ccsc2ccccc12
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[c:5]:[#16;a:6]>>[#16;a:6]:[c:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
54
[{"value": 54.0, "product": "C(=O)(O)C1=C(SC2=C(C1=O)C=C(C(=C2F)F)F)SC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 53.6, "product": "C(=O)(O)C1=C(SC2=C(C1=O)C=C(C(=C2F)F)F)SC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
3
HOUR
A mixture of 300 mg (0.897 mmol) of the compound of Example 111, 0.54 ml of acetic acid, 0.072 ml of concentrated sulfuric acid and 0.36 ml of water was stirred for 3 hours at 100° C. After cooling by allowing to stand, the crystals deposited were collected by filtration, washed with water, and dried to obtain 147 mg (...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1csc2ccccc2c1
Other
O
100
3
CCOC(=O)c1c(SC)sc2c(F)c(F)c(F)cc2c1=O>O>CSc1sc2c(F)c(F)c(F)cc2c(=O)c1C(=O)O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-650824152b5742c386e87f846affa28e
COc1ccc(CCl)cc1.CSc1sc2c(F)c(F)c(F)cc2c(=O)c1C(=O)O>>COc1ccc(COC(=O)c2c(SC)sc3c(F)c(F)c(F)cc3c2=O)cc1
C(=O)(O)C1=C(SC2=C(C1=O)C=C(C(=C2F)F)F)SC.COC1=CC=C(CCl)C=C1.C(C)N(CC)CC.[I-].[Na+]>>COC1=CC=C(COC(=O)C2=C(SC3=C(C2=O)C=C(C(=C3F)F)F)SC)C=C1
Cl[CH2:7][c:6]1[cH:5][cH:4][c:3]([O:2][CH3:1])[cH:28][cH:27]1.[OH:8][C:9](=[O:10])[c:11]1[c:12]([S:13][CH3:14])[s:15][c:16]2[c:17]([F:18])[c:19]([F:20])[c:21]([F:22])[cH:23][c:24]2[c:25]1=[O:26]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][c:6]([CH2:7][O:8][C:9](=[O:10])[c:11]2[c:12]([S:13][CH3:14])[s:15][c:16]3[c:17]([F:18])[c:19]...
COc1ccc(CCl)cc1.CSc1sc2c(F)c(F)c(F)cc2c(=O)c1C(=O)O
COc1ccc(COC(=O)c2c(SC)sc3c(F)c(F)c(F)cc3c2=O)cc1
null
null
C(Cl)(Cl)Cl
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
06c4f868ad4646eea8208ecb83f54ca035dd62d04f0d8101641a4f487f2c695c
8446834f0edd1e71a2dcaffc09b80c7367abf3407263a8998354a2d20c1766bb
O=C(OCc1ccccc1)c1csc2ccccc2c1=O
Cl-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[#16;a:5]:[c:6]:[c:7]-[C:8](=[O;D1;H0:9])-[OH;D1;+0:10]>>[#16;a:5]:[c:6]:[c:7]-[C:8](=[O;D1;H0:9])-[O;H0;D2;+0:10]-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
32.4
[{"value": 32.0, "product": "COC1=CC=C(COC(=O)C2=C(SC3=C(C2=O)C=C(C(=C3F)F)F)SC)C=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 32.4, "product": "COC1=CC=C(COC(=O)C2=C(SC3=C(C2=O)C=C(C(=C3F)F)F)SC)C=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
5
HOUR
To a suspension of 50 mg (0.163 mmol) of the compound of Example 112 in 0.2 ml of chloroform were added 30.7 mg (0.196 mmol) of p-methoxybenzyl chloride, 16.5 mg (0.163 mmol) of triethylamine and 29.4 mg (0.196 mmol) of sodium iodide, and the mixture was stirred for 5 hours at room temperature, which was poured into ic...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Carboxylic acid
Ester
null
null
c1ccccc1.c1csc2ccccc2c1
HCl
C(Cl)(Cl)Cl
null
5
COc1ccc(CCl)cc1.CSc1sc2c(F)c(F)c(F)cc2c(=O)c1C(=O)O>C(Cl)(Cl)Cl>COc1ccc(COC(=O)c2c(SC)sc3c(F)c(F)c(F)cc3c2=O)cc1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-65534682ee6b4b1b840f36d71ebb8513
Nc1cc([N+](=O)[O-])ccc1C=O>>Nc1ccc(C=O)c(N)c1
NC1=C(C=O)C=CC(=C1)[N+](=O)[O-]>>NC1=C(C=O)C=CC(=C1)N
O=[N+:1]([O-])[c:2]1[cH:3][cH:4][c:5]([CH:6]=[O:7])[c:8]([NH2:9])[cH:10]1>>[NH2:1][c:2]1[cH:3][cH:4][c:5]([CH:6]=[O:7])[c:8]([NH2:9])[cH:10]1
Nc1cc([N+](=O)[O-])ccc1C=O
Nc1ccc(C=O)c(N)c1
null
[Pd]
null
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
c1ccccc1
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]>>[NH2;D1;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
null
null
In a manner similar to that described for 10-nitro-20(RS)- and 10-nitro-20(S)-camptothecin, a mixture of 2-amino-4-nitrobenzaldehyde is treated with the tricyclic ketone 11 yielding 11-nitro-20(RS)- or 11-nitro-20(S)-camptothecin which in turn is reduced to 11-amino compound camptothecin by palladium/carbon. Alternativ...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1
Other
[Pd]
null
null
Nc1cc([N+](=O)[O-])ccc1C=O>[Pd]>Nc1ccc(C=O)c(N)c1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-06f5c13d44cb4445b1c0ad64e71f27b9
CCOC(=O)C1CCCN(C(=O)OC(C)(C)C)C1.ClCCCBr>>CCOC(=O)C12CCCN(CCC1)C2
C(C)OC(=O)C1CN(CCC1)C(=O)OC(C)(C)C.C(C)(C)[N-]C(C)C.[Li+].O1CCCC1.BrCCCCl>>C(C)OC(=O)C12CCCN(CCC1)C2
CC(C)(C)OC(=O)[N:10]1[CH2:9][CH2:8][CH2:7][CH:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[CH2:14]1.Cl[CH2:13][CH2:12][CH2:11]Br>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[C:6]12[CH2:7][CH2:8][CH2:9][N:10]([CH2:11][CH2:12][CH2:13]1)[CH2:14]2
CCOC(=O)C1CCCN(C(=O)OC(C)(C)C)C1.ClCCCBr
CCOC(=O)C12CCCN(CCC1)C2
null
null
O1CCCC1
Heteroatom Alkylation and Arylation
OtherReaction
f0e6b5f83e3ba6a6fa98f66780a4137e5da2f647c6fa968f1e5e4d5e42ebd8b8
3f5dc1d93193b3e0a3d863cd886d5171d5b06000b75ac28593dfbd0f57ac702a
C1CC2CCCN(C1)C2
Br-[CH2;D2;+0:1]-[C:2]-[CH2;D2;+0:3]-Cl.C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:4]1-[C:5]-[CH;D3;+0:6](-[C:7](=[O;D1;H0:8])-[#8:9]-[C:10])-[C:11]-[C:12]-[C:13]-1>>[C:10]-[#8:9]-[C:7](=[O;D1;H0:8])-[C;H0;D4;+0:6]12-[C:5]-[N;H0;D3;+0:4](-[C:13]-[C:12]-[C:11]-1)-[CH2;D2;+0:1]-[C:2]-[CH2;D2;+0:3]-2
73
[{"value": 73.0, "product": "C(C)OC(=O)C12CCCN(CCC1)C2", "details": "PERCENTYIELD", "is_desired": false}, {"value": 73.0, "product": "C(C)OC(=O)C12CCCN(CCC1)C2", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-35
CELSIUS
1
HOUR
A cooled (-50° C.) solution of 1,3-piperidinedicarboxylic acid 1-(1,1-dimethylethyl) 3-ethyl ester (12.9 g, 50 mmol) in anhydrous tetrahydrofuran (60 mL) was treated (via syringe) with 1.15N lithium diisopropylamide/tetrahydorfuran (52 mmol), stirred for one hour at -15°±5° C., cooled (-35° C.), treated with 1-bromo-3-...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary halide.Carbamic ester.Ester.Ether.Boc
Ester.Tertiary amine
C1CC[NH]CC1
C1CC2CCCN(C1)C2
C1CC2CCCN(C1)C2
HCl.Br-
O1CCCC1
-35
1
CCOC(=O)C1CCCN(C(=O)OC(C)(C)C)C1.ClCCCBr>O1CCCC1>CCOC(=O)C12CCCN(CCC1)C2
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-3f6f7292f4214dacbbc44e42e9963d38
CCOC(=O)C12CCCN(CC1)C2>>OCC12CCCN(CC1)C2
[H-].[Al+3].[Li+].[H-].[H-].[H-].O1CCCC1.O.[OH-].[Na+].O.C(C)OC(=O)C12CCCN(CC1)C2>>N12CCCC(CC1)(C2)CO
CCO[C:2](=[O:1])[C:3]12[CH2:4][CH2:5][CH2:6][N:7]([CH2:8][CH2:9]1)[CH2:10]2>>[OH:1][CH2:2][C:3]12[CH2:4][CH2:5][CH2:6][N:7]([CH2:8][CH2:9]1)[CH2:10]2
CCOC(=O)C12CCCN(CC1)C2
OCC12CCCN(CC1)C2
null
null
O1CCCC1
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
C1CC2CCN(C1)C2
C-C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[C:3](-[C:4])(-[C:5])-[C:6]-[#7:7]>>[#7:7]-[C:6]-[C:3](-[CH2;D2;+0:1]-[OH;D1;+0:2])(-[C:4])-[C:5]
null
[]
null
null
30
MINUTE
A cooled (0° C.) solution of 1.0N lithium aluminum hydride/tetrahydrofuran (55 mL, 55 mmol) under nitrogen was treated dropwise with a solution of 1-azabicyclo[3.2.1]octane-5-carboxylic acid ethyl ester (9.17 g, 50 mmol) in anhydrous tetrahydrofuran (20 mL), stirred for 30 minutes at room temperature, refluxed for one ...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
C1CC2CCN(C1)C2
HO-
O1CCCC1
null
0.5
CCOC(=O)C12CCCN(CC1)C2>O1CCCC1>OCC12CCCN(CC1)C2
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-724adf2a51f8489d97c3c818d08a607f
CCOC(=O)C12CCCN(CCC1)C2>>OCC12CCCN(CCC1)C2
O.[OH-].[Na+].O.C(C)OC(=O)C12CCCN(CCC1)C2.[H-].[Al+3].[Li+].[H-].[H-].[H-].O1CCCC1>>N12CCCC(CCC1)(C2)CO
CCO[C:2](=[O:1])[C:3]12[CH2:4][CH2:5][CH2:6][N:7]([CH2:8][CH2:9][CH2:10]1)[CH2:11]2>>[OH:1][CH2:2][C:3]12[CH2:4][CH2:5][CH2:6][N:7]([CH2:8][CH2:9][CH2:10]1)[CH2:11]2
CCOC(=O)C12CCCN(CCC1)C2
OCC12CCCN(CCC1)C2
null
null
O1CCCC1
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
C1CC2CCCN(C1)C2
C-C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[C:3](-[C:4])(-[C:5])-[C:6]-[#7:7]>>[#7:7]-[C:6]-[C:3](-[CH2;D2;+0:1]-[OH;D1;+0:2])(-[C:4])-[C:5]
98
[{"value": 98.0, "product": "N12CCCC(CCC1)(C2)CO", "details": "PERCENTYIELD", "is_desired": false}, {"value": 97.9, "product": "N12CCCC(CCC1)(C2)CO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
A solution of 1-azabicyclo[3.3.1]nonane-5-carboxylic acid ethyl ester (9.08 g, 46 mmol) in anhydrous tetrahydrofuran (25 mL) was added dropwise to a cooled (-10° C.) solution of 1.0N lithium aluminum hydride/tetrahydrofuran (50 mL, 50 mmol) in a 3-neck, 250-mL flask under nitrogen at a rate to keep the reaction tempera...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
C1CC2CCCN(C1)C2
HO-
O1CCCC1
null
0.25
CCOC(=O)C12CCCN(CCC1)C2>O1CCCC1>OCC12CCCN(CCC1)C2
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-a207e32502304f06a21da6f82ecce891
NO.OCC12CCCN(CCC1)C2>>ON=CC12CCCN(CCC1)C2
CS(=O)C.Cl.NO.C[O-].[Na+].CO.C[O-].[Na+].N12CCCC(CCC1)(C2)CO.C(C(=O)Cl)(=O)Cl>>N12CCCC(CCC1)(C2)C=NO
[OH:1][NH2:2].O[CH2:3][C:4]12[CH2:5][CH2:6][CH2:7][N:8]([CH2:9][CH2:10][CH2:11]1)[CH2:12]2>>[OH:1][N:2]=[CH:3][C:4]12[CH2:5][CH2:6][CH2:7][N:8]([CH2:9][CH2:10][CH2:11]1)[CH2:12]2
NO.OCC12CCCN(CCC1)C2
ON=CC12CCCN(CCC1)C2
null
null
C(Cl)Cl.C(C)N(CC)CC
Heteroatom Alkylation and Arylation
OtherReaction
6e036145121e74fec2a8b1c98baa36a6154968367991affa3e65663e26a5dd0f
5b1c2692f91b6028790c632ddd5f7bb4ef9cf197bdd095bee03fa688aa8c3259
C1CC2CCCN(C1)C2
O-[CH2;D2;+0:1]-[C:2](-[C:3])(-[C:4])-[C:5]-[#7:6].[NH2;D1;+0:7]-[O;D1;H1:8]>>[#7:6]-[C:5]-[C:2](-[CH;D2;+0:1]=[N;H0;D2;+0:7]-[O;D1;H1:8])(-[C:3])-[C:4]
60
[{"value": 60.0, "product": "N12CCCC(CCC1)(C2)C=NO", "details": "PERCENTYIELD", "is_desired": false}, {"value": 59.9, "product": "N12CCCC(CCC1)(C2)C=NO", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
A cooled (-65° C.) solution of oxalyl chloride (5.3 mL, 60 mmol) in anhydrous methylene chloride (100 mL) under nitrogen was treated dropwise with anhydrous dimethylsulfoxide (0.60 g, 120 mmol) in methylene chloride (30 mL) at a rate to keep the reaction temperature below -60° C. After 30 minutes at -65° C., a solution...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Primary amine
Oxime
null
null
C1CC2CCCN(C1)C2
HO-
C(Cl)Cl.C(C)N(CC)CC
null
0.5
NO.OCC12CCCN(CCC1)C2>C(Cl)Cl.C(C)N(CC)CC>ON=CC12CCCN(CCC1)C2
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-37ba75b1b1944de596d5785b37bb6bfe
COC(=O)C12CCCN(CCC1)C2.N>>NC(=O)C12CCCN(CCC1)C2
COC(=O)C12CCCN(CCC1)C2.N>>N12CCCC(CCC1)(C2)C(=O)N
CO[C:2](=[O:3])[C:4]12[CH2:5][CH2:6][CH2:7][N:8]([CH2:9][CH2:10][CH2:11]1)[CH2:12]2.[NH3:1]>>[NH2:1][C:2](=[O:3])[C:4]12[CH2:5][CH2:6][CH2:7][N:8]([CH2:9][CH2:10][CH2:11]1)[CH2:12]2
COC(=O)C12CCCN(CCC1)C2.N
NC(=O)C12CCCN(CCC1)C2
null
C[O-].[Na+].CO
CO
Acylation
OtherReaction
d5b10d4f469e7a196a3b04a6a9e159a7d90514b6df5b50c1197d4b1b774c04e1
adc0ef6f6c1340dd2dbab737c85bf17fc842769181c5db1a2b4f82b391b28f9f
C1CC2CCCN(C1)C2
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])(-[C:5])-[C:6]-[#7:7].[NH3;D0;+0:8]>>[#7:7]-[C:6]-[C:3](-[C;H0;D3;+0:1](-[NH2;D1;+0:8])=[O;D1;H0:2])(-[C:4])-[C:5]
38
[{"value": 38.0, "product": "N12CCCC(CCC1)(C2)C(=O)N", "details": "PERCENTYIELD", "is_desired": false}]
150
CELSIUS
null
null
A solution of 1-azabicyclo[3.3.1]nonane-5-carboxylic acid methyl ester (1.83 g, 10 mmol) in ammonia (50 mL) and methanol (20 mL) was sealed in a bomb and heated at 120°-130° C. for 36 hours (gas chromatography indicated that the reaction was incomplete). Three drops of 25% sodium methoxide/methanol were added, and the ...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary amide
null
null
C1CC2CCCN(C1)C2
HO-
C[O-].[Na+].CO.CO
150
null
COC(=O)C12CCCN(CCC1)C2.N>C[O-].[Na+].CO.CO>NC(=O)C12CCCN(CCC1)C2
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-0445a3a91b3b46b584c36be6a9648625
NC(=O)C12CCCN(CCC1)C2>>NCC12CCCN(CCC1)C2
O.[OH-].[Na+].O.N12CCCC(CCC1)(C2)C(=O)N.[H-].[Al+3].[Li+].[H-].[H-].[H-].O1CCCC1>>N12CCCC(CCC1)(C2)CN
O=[C:2]([NH2:1])[C:3]12[CH2:4][CH2:5][CH2:6][N:7]([CH2:8][CH2:9][CH2:10]1)[CH2:11]2>>[NH2:1][CH2:2][C:3]12[CH2:4][CH2:5][CH2:6][N:7]([CH2:8][CH2:9][CH2:10]1)[CH2:11]2
NC(=O)C12CCCN(CCC1)C2
NCC12CCCN(CCC1)C2
null
null
CCOCC.O1CCCC1
Reduction
Reduction of primary amides to amines
71f4ab6e4ff9fd6ad8fb6a6879cdc6c258d35bb85b9b40ad2783b874bf909ba4
8776a0c3e2f32dafe87200a597cd55df0b01414bf133bdc9f8f7e1171014bfad
C1CC2CCCN(C1)C2
O=[C;H0;D3;+0:1](-[N;D1;H2:2])-[C:3](-[C:4])(-[C:5])-[C:6]-[#7:7]>>[#7:7]-[C:6]-[C:3](-[CH2;D2;+0:1]-[N;D1;H2:2])(-[C:4])-[C:5]
77
[{"value": 77.0, "product": "N12CCCC(CCC1)(C2)CN", "details": "PERCENTYIELD", "is_desired": false}, {"value": 76.9, "product": "N12CCCC(CCC1)(C2)CN", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
null
null
A suspension of 1-azabicyclo[3.3.1]nonane-5-carboxamide (1.80 g, 10.7 mmol) in anhydrous tetrahydrofuran (10 mL) under nitrogen was treated (via syringe) with 1.0N lithium aluminum hydride/tetrahydrofuran (25 mL, 25 mmol), and the mixture was refluxed for 4 hours and cooled (0° C.). The mixture was treated carefully dr...
10.6084/m9.figshare.5104873.v1
null
Primary amide
null
null
null
C1CC2CCCN(C1)C2
Other
CCOCC.O1CCCC1
0
null
NC(=O)C12CCCN(CCC1)C2>CCOCC.O1CCCC1>NCC12CCCN(CCC1)C2
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-042aee9b85f3448db5bd4bc2f82e203c
COS(=O)(=O)OC.O=C(O)c1c[nH]c2ccccc12>>Cn1cc(C(=O)O)c2ccccc21
[H-].[Na+].N1C=C(C2=CC=CC=C12)C(=O)O.[OH-].[Na+].COS(=O)(=O)OC>>CN1C=C(C2=CC=CC=C12)C(=O)O
COS(=O)(=O)O[CH3:1].[nH:2]1[cH:3][c:4]([C:5](=[O:6])[OH:7])[c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]12>>[CH3:1][n:2]1[cH:3][c:4]([C:5](=[O:6])[OH:7])[c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]12
COS(=O)(=O)OC.O=C(O)c1c[nH]c2ccccc12
Cn1cc(C(=O)O)c2ccccc21
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
N-methylation
5ce73e9bd608d5491381e563c654ad03f655de6d7aa46423d6263e854c49919a
7a358c636daddc97c1fb4c29f378044d7eac3f01815d9966e599841f642d631a
c1ccc2[nH]ccc2c1
C-O-S(=O)(=O)-O-[CH3;D1;+0:1].[O;D1;H0:2]=[C:3](-[O;D1;H1:4])-[c:5]1:[c:6]:[nH;D2;+0:7]:[c:8](:[c:9]):[c:10]:1>>[CH3;D1;+0:1]-[n;H0;D3;+0:7]1:[c:6]:[c:5](-[C:3](=[O;D1;H0:2])-[O;D1;H1:4]):[c:10]:[c:8]:1:[c:9]
75.3
[{"value": 75.0, "product": "CN1C=C(C2=CC=CC=C12)C(=O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 75.3, "product": "CN1C=C(C2=CC=CC=C12)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
100
CELSIUS
30
MINUTE
A cooled (0° C.) suspension of 60% sodium hydride-oil dispersion (0.96 g, 24 mmol) in anhydrous N,N-dimethylformamide (15 mL) under nitrogen was treated in portions with indole-3-carboxylic acid (1.62 g, 10 mmol), and the mixture was stirred at 45°±5° C. for 30 minutes. Dimethylsulfate (3.03 g, 24 mmol) was added, and ...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ccc2[nH]ccc2c1
c1c[nH]c2ccccc12
c1c[nH]c2ccccc12
HO-
CN(C=O)C
100
0.5
COS(=O)(=O)OC.O=C(O)c1c[nH]c2ccccc12>CN(C=O)C>Cn1cc(C(=O)O)c2ccccc21
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-76e193244c0648009545e2db9839eabd
COC(=O)c1nn(C)c2ccccc12>>Cn1nc(C(=O)O)c2ccccc21
Cl.CN1N=C(C2=CC=CC=C12)C(=O)OC.[OH-].[Na+]>>CN1N=C(C2=CC=CC=C12)C(=O)O
C[O:7][C:5]([c:4]1[n:3][n:2]([CH3:1])[c:13]2[c:8]1[cH:9][cH:10][cH:11][cH:12]2)=[O:6]>>[CH3:1][n:2]1[n:3][c:4]([C:5](=[O:6])[OH:7])[c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]12
COC(=O)c1nn(C)c2ccccc12
Cn1nc(C(=O)O)c2ccccc21
null
null
CO.O
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc2[nH]ncc2c1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]:[#7;a:5]:[#7;a:6]>>[#7;a:6]:[#7;a:5]:[c:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1]
92.1
[{"value": 92.0, "product": "CN1N=C(C2=CC=CC=C12)C(=O)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 92.1, "product": "CN1N=C(C2=CC=CC=C12)C(=O)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 1-methylindazole-3-carboxylic acid, methyl ester (1.00 g, 0.0053 mol) was stirred in a mixture of methanol (10 mL)/2N NaOH solution (120 mL) at reflux temperature for 2 hours. After cooling, the mixture was diluted with water (100 mL) and acidified with 6N HCl solution. The white solid that formed was col...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1n[nH]c2ccccc12
Other
CO.O
null
null
COC(=O)c1nn(C)c2ccccc12>CO.O>Cn1nc(C(=O)O)c2ccccc21
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-b8ad3a760b1242ffb810507057579d5e
COc1cc(N)c(Cl)cc1C(=O)O>>Nc1cc(O)c(C(=O)O)cc1Cl
[H-].[Na+].C(C)S.NC1=CC(=C(C(=O)O)C=C1Cl)OC>>NC1=CC(=C(C(=O)O)C=C1Cl)O
C[O:5][c:4]1[cH:3][c:2]([NH2:1])[c:11]([Cl:12])[cH:10][c:6]1[C:7](=[O:8])[OH:9]>>[NH2:1][c:2]1[cH:3][c:4]([OH:5])[c:6]([C:7](=[O:8])[OH:9])[cH:10][c:11]1[Cl:12]
COc1cc(N)c(Cl)cc1C(=O)O
Nc1cc(O)c(C(=O)O)cc1Cl
null
null
CN(C=O)C
Deprotection
Cleavage of methoxy ethers to alcohols
c5320c7dfa4f544d4900efcae9b3262bf0d5286bcf39c86109232351f35b23d5
26a36596df80ec137b0e8087297418351c93c32819177f680675220622f215d4
c1ccccc1
C-[O;H0;D2;+0:1]-[c:2](:[c:3]):[c:4]-[C:5](=[O;D1;H0:6])-[O;D1;H1:7]>>[O;D1;H0:6]=[C:5](-[O;D1;H1:7])-[c:4]:[c:2](-[OH;D1;+0:1]):[c:3]
83.4
[{"value": 83.0, "product": "NC1=CC(=C(C(=O)O)C=C1Cl)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 83.4, "product": "NC1=CC(=C(C(=O)O)C=C1Cl)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
A cooled (5° C.) suspension of 60% sodium hydride/oil dispersion (20.0 g, 0.50 mole) in anhydrous dimethylformamide (300 mL) under nitrogen was treated slowly dropwise with ethyl mercaptan (18.7 g, 0.30 mole) so as to maintain a pot temperature below 15° C., then stirred at room temperature for 15 minutes, cooled (5° C...
10.6084/m9.figshare.5104873.v1
null
Ether
Aromatic alcohol
null
null
c1ccccc1
Other
CN(C=O)C
null
0.25
COc1cc(N)c(Cl)cc1C(=O)O>CN(C=O)C>Nc1cc(O)c(C(=O)O)cc1Cl
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-5ef4854df60141d78ca949d2c8047a2b
CO.Nc1cc(O)c(C(=O)O)cc1Cl>>COC(=O)c1cc(Cl)c(N)cc1O
S(=O)(=O)(OC)OC.NC1=CC(=C(C(=O)O)C=C1Cl)O.C[O-].[Na+].CO>>NC1=CC(=C(C(=O)OC)C=C1Cl)O
O[CH3:1].[OH:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([Cl:8])[c:9]([NH2:10])[cH:11][c:12]1[OH:13]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][c:7]([Cl:8])[c:9]([NH2:10])[cH:11][c:12]1[OH:13]
CO.Nc1cc(O)c(C(=O)O)cc1Cl
COC(=O)c1cc(Cl)c(N)cc1O
null
null
CO.O
Heteroatom Alkylation and Arylation
Esterification of Carboxylic Acids
961bfcd5802efbb4a2d5a1e38cbfb6654b5b78f769c3570df49b858a6f105ab6
0a622556a49b258b9020bd3a5bdd1fa9237e7093cf9b09de3a6b575ffe935dcd
c1ccccc1
O-[CH3;D1;+0:1].[O;D1;H0:2]=[C:3](-[OH;D1;+0:4])-[c:5]>>[CH3;D1;+0:1]-[O;H0;D2;+0:4]-[C:3](=[O;D1;H0:2])-[c:5]
87
[{"value": 87.0, "product": "NC1=CC(=C(C(=O)OC)C=C1Cl)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 86.8, "product": "NC1=CC(=C(C(=O)OC)C=C1Cl)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
A solution of 4-amino-5-chloro-2-hydroxybenzoic acid (1.88 g, 10 mmol) in absolute methanol (20 mL) was treated with 25% sodium methoxide/methanol (2.16 g, 10 mmol), stirred for 30 minutes, and concentrated in vacuo. The solid residue was taken up in anhydrous acetone (30 mL), treated with dimethyl sulfate (1.64 g, 13 ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Methanol
Ester
null
null
c1ccccc1
HO-
CO.O
null
0.5
CO.Nc1cc(O)c(C(=O)O)cc1Cl>CO.O>COC(=O)c1cc(Cl)c(N)cc1O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-4901bf8f54dc48a7ac09c0ddf6fdf741
COC(=O)c1cc(Cl)c(N)cc1O.COCCBr>>COCCOc1cc(N)c(Cl)cc1C(=O)OC
O.COC(C1=C(C=C(C(=C1)Cl)N)O)=O.[H-].[Na+].COCCBr>>COC(C1=C(C=C(C(=C1)Cl)N)OCCOC)=O
[OH:5][c:6]1[cH:7][c:8]([NH2:9])[c:10]([Cl:11])[cH:12][c:13]1[C:14](=[O:15])[O:16][CH3:17].Br[CH2:4][CH2:3][O:2][CH3:1]>>[CH3:1][O:2][CH2:3][CH2:4][O:5][c:6]1[cH:7][c:8]([NH2:9])[c:10]([Cl:11])[cH:12][c:13]1[C:14](=[O:15])[O:16][CH3:17]
COC(=O)c1cc(Cl)c(N)cc1O.COCCBr
COCCOc1cc(N)c(Cl)cc1C(=O)OC
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
7e1040116e3a4cf0e8ec5cc7865388d9cd0efabce6d320a1c25a36e411018d8b
d5f4610d46ccc0478471c5bc0fb862644eaf764bbc5d93badb39d54f6ec8e0a5
c1ccccc1
Br-[CH2;D2;+0:1]-[C:2]-[#8:3].[#8:4]-[C:5](=[O;D1;H0:6])-[c:7]:[c:8](-[OH;D1;+0:9]):[c:10]>>[#8:4]-[C:5](=[O;D1;H0:6])-[c:7]:[c:8](-[O;H0;D2;+0:9]-[CH2;D2;+0:1]-[C:2]-[#8:3]):[c:10]
53
[{"value": 53.0, "product": "COC(C1=C(C=C(C(=C1)Cl)N)OCCOC)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 52.9, "product": "COC(C1=C(C=C(C(=C1)Cl)N)OCCOC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
A suspension of 60% sodium hydride/oil dispersion (1.00 g, 25 mmol) in anhydrous dimethylformamide (40 mL) under nitrogen was treated with 4-amino-5-chloro-2-hydroxybenzoic acid methyl ester (4.03 g, 20 mmol), stirred for 30 minutes, then treated with 2-bromoethyl methyl ether (3.48 g, 25 mmol). The mixture was heated ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic alcohol
Ether
null
null
c1ccccc1
HBr
CN(C=O)C
null
0.5
COC(=O)c1cc(Cl)c(N)cc1O.COCCBr>CN(C=O)C>COCCOc1cc(N)c(Cl)cc1C(=O)OC
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-1be6548ad9b94f2f8afd6c1d75cd9889
COCCOc1cc(N)c(Cl)cc1C(=O)OC>>COCCOc1cc(N)c(Cl)cc1C(=O)O
COC(C1=C(C=C(C(=C1)Cl)N)OCCOC)=O.[OH-].[Na+].O>>NC1=CC(=C(C(=O)O)C=C1Cl)OCCOC
C[O:16][C:14]([c:13]1[c:6]([O:5][CH2:4][CH2:3][O:2][CH3:1])[cH:7][c:8]([NH2:9])[c:10]([Cl:11])[cH:12]1)=[O:15]>>[CH3:1][O:2][CH2:3][CH2:4][O:5][c:6]1[cH:7][c:8]([NH2:9])[c:10]([Cl:11])[cH:12][c:13]1[C:14](=[O:15])[OH:16]
COCCOc1cc(N)c(Cl)cc1C(=O)OC
COCCOc1cc(N)c(Cl)cc1C(=O)O
null
null
C(C)O
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccccc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]
78
[{"value": 75.0, "product": "NC1=CC(=C(C(=O)O)C=C1Cl)OCCOC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 78.0, "product": "NC1=CC(=C(C(=O)O)C=C1Cl)OCCOC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 4-amino-5-chloro-2-(2-methoxyethoxy)benzoic acid methyl ester (2.75 g, 10.6 mmol) in 95% ethanol (20 mL) was treated with 50% sodium hydroxide (10 mL) and water (10 mL), and refluxed for one hour. The ethanol was removed in vacuo and replaced with water. The aqueous solution was extracted with ether (20 m...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1
Other
C(C)O
null
null
COCCOc1cc(N)c(Cl)cc1C(=O)OC>C(C)O>COCCOc1cc(N)c(Cl)cc1C(=O)O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-55c482b078c24bb4b5e2982805ae9829
COC(=O)c1ccc(N)cc1.CS(=O)(=O)Cl>>COC(=O)c1ccc(NS(C)(=O)=O)cc1
Cl.CS(=O)(=O)Cl.N1=CC=CC=C1.NC1=CC=C(C(=O)OC)C=C1>>COC(C1=CC=C(C=C1)NS(=O)(=O)C)=O
[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([NH2:9])[cH:14][cH:15]1.Cl[S:10]([CH3:11])(=[O:12])=[O:13]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([NH:9][S:10]([CH3:11])(=[O:12])=[O:13])[cH:14][cH:15]1
COC(=O)c1ccc(N)cc1.CS(=O)(=O)Cl
COC(=O)c1ccc(NS(C)(=O)=O)cc1
null
null
C(Cl)Cl
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
c1ccccc1
Cl-[S;H0;D4;+0:1](-[C;D1;H3:2])(=[O;D1;H0:3])=[O;D1;H0:4].[NH2;D1;+0:5]-[c:6](:[c:7]):[c:8]>>[C;D1;H3:2]-[S;H0;D4;+0:1](=[O;D1;H0:3])(=[O;D1;H0:4])-[NH;D2;+0:5]-[c:6](:[c:7]):[c:8]
95.2
[{"value": 91.5, "product": "COC(C1=CC=C(C=C1)NS(=O)(=O)C)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 95.2, "product": "COC(C1=CC=C(C=C1)NS(=O)(=O)C)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
A solution of methanesulfonyl chloride (15.2 g, 132 mmol) in methylene chloride (50 mL) was added dropwise to a stirring slurry of pyridine (41.8 g, 529 mmol) and methyl 4-aminobenzoate (20.0 g, 132 mmol) in methylene chloride (110 mL) cooled by a dry ice/acetone bath. The reaction mixture was allowed to warm to ambien...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
c1ccccc1
HCl
C(Cl)Cl
null
8
COC(=O)c1ccc(N)cc1.CS(=O)(=O)Cl>C(Cl)Cl>COC(=O)c1ccc(NS(C)(=O)=O)cc1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-d21c947da703415f83c8dca17871db03
CCN(CC)C(=O)COc1cc(N)c(Cl)cc1C(=O)OC>>CCN(CC)C(=O)COc1cc(N)c(Cl)cc1C(=O)O
Cl.[OH-].[Na+].NC1=CC(=C(C(=O)OC)C=C1Cl)OCC(=O)N(CC)CC.CO>>NC1=CC(=C(C(=O)O)C=C1Cl)OCC(=O)N(CC)CC
C[O:20][C:18]([c:17]1[c:10]([O:9][CH2:8][C:6]([N:3]([CH2:2][CH3:1])[CH2:4][CH3:5])=[O:7])[cH:11][c:12]([NH2:13])[c:14]([Cl:15])[cH:16]1)=[O:19]>>[CH3:1][CH2:2][N:3]([CH2:4][CH3:5])[C:6](=[O:7])[CH2:8][O:9][c:10]1[cH:11][c:12]([NH2:13])[c:14]([Cl:15])[cH:16][c:17]1[C:18](=[O:19])[OH:20]
CCN(CC)C(=O)COc1cc(N)c(Cl)cc1C(=O)OC
CCN(CC)C(=O)COc1cc(N)c(Cl)cc1C(=O)O
null
null
O
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccccc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]
68.1
[{"value": 68.0, "product": "NC1=CC(=C(C(=O)O)C=C1Cl)OCC(=O)N(CC)CC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 68.1, "product": "NC1=CC(=C(C(=O)O)C=C1Cl)OCC(=O)N(CC)CC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
60
CELSIUS
null
null
A solution of 4-amino-5-chloro-2-[2-(diethylamino)-2-oxoethoxy]benzoic acid, methyl ester (7.87 g, 25 mmol) in water (70 g) containing methanol (40 g) was treated with 50% sodium hydroxide (10 g) and heated to 60° C. for 30 minutes. The mixture was neutralized with 3N HCl until a precipitate formed (pH 3), and the soli...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1
Other
O
60
null
CCN(CC)C(=O)COc1cc(N)c(Cl)cc1C(=O)OC>O>CCN(CC)C(=O)COc1cc(N)c(Cl)cc1C(=O)O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-257d8a8cf6e94ad4a79fa20e809fe6eb
C=CCBr.COC(=O)c1cc(Cl)c(N)cc1O>>C=CCOc1cc(N)c(Cl)cc1C(=O)O
O.COC(C1=C(C=C(C(=C1)Cl)N)O)=O.[H-].[Na+].C(C=C)Br>>NC1=CC(=C(C(=O)O)C=C1Cl)OCC=C
Br[CH2:3][CH:2]=[CH2:1].C[O:15][C:13]([c:12]1[c:5]([OH:4])[cH:6][c:7]([NH2:8])[c:9]([Cl:10])[cH:11]1)=[O:14]>>[CH2:1]=[CH:2][CH2:3][O:4][c:5]1[cH:6][c:7]([NH2:8])[c:9]([Cl:10])[cH:11][c:12]1[C:13](=[O:14])[OH:15]
C=CCBr.COC(=O)c1cc(Cl)c(N)cc1O
C=CCOc1cc(N)c(Cl)cc1C(=O)O
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
OtherReaction
c47049bacd28cc701f2e77df376a2fcefecd5392e081f9a62473cff265d23a8c
017337a0828c32d10d28543003ae15a8b492b5e2f69019c65a4461eabc617d95
c1ccccc1
Br-[CH2;D2;+0:1]-[C:2]=[C;D1;H2:3].C-[O;H0;D2;+0:4]-[C:5](=[O;D1;H0:6])-[c:7]:[c:8](-[OH;D1;+0:9]):[c:10]>>[C;D1;H2:3]=[C:2]-[CH2;D2;+0:1]-[O;H0;D2;+0:9]-[c:8](:[c:10]):[c:7]-[C:5](=[O;D1;H0:6])-[OH;D1;+0:4]
62.2
[{"value": 62.2, "product": "NC1=CC(=C(C(=O)O)C=C1Cl)OCC=C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 62.2, "product": "NC1=CC(=C(C(=O)O)C=C1Cl)OCC=C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
A suspension of 60% sodium hydride/oil dispersion (1.52 g, 38 mmol) in anhydrous dimethylformamide (50 mL) under nitrogen was treated in portions with 4-amino-5-chloro-2-hydroxybenzoic acid methyl ester (6.05 g, 30 mmol), stirred at room temperature for 30 minutes, and treated with allyl bromide (4.60 g, 38 mmol). The ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester.Aromatic alcohol
Carboxylic acid.Ether
null
null
c1ccccc1
HBr
CN(C=O)C
null
0.5
C=CCBr.COC(=O)c1cc(Cl)c(N)cc1O>CN(C=O)C>C=CCOc1cc(N)c(Cl)cc1C(=O)O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-4a61892e548641678c1f2f77ac5daff8
CSCCCl.Nc1cc(O)c(C(=O)O)cc1Cl>>CSCCOc1cc(N)c(Cl)cc1C(=O)O
[H-].[Na+].NC1=CC(=C(C(=O)O)C=C1Cl)O.ClCCSC>>NC1=CC(=C(C(=O)O)C=C1Cl)OCCSC
Cl[CH2:4][CH2:3][S:2][CH3:1].[OH:5][c:6]1[cH:7][c:8]([NH2:9])[c:10]([Cl:11])[cH:12][c:13]1[C:14](=[O:15])[OH:16]>>[CH3:1][S:2][CH2:3][CH2:4][O:5][c:6]1[cH:7][c:8]([NH2:9])[c:10]([Cl:11])[cH:12][c:13]1[C:14](=[O:15])[OH:16]
CSCCCl.Nc1cc(O)c(C(=O)O)cc1Cl
CSCCOc1cc(N)c(Cl)cc1C(=O)O
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
7e1040116e3a4cf0e8ec5cc7865388d9cd0efabce6d320a1c25a36e411018d8b
d5f4610d46ccc0478471c5bc0fb862644eaf764bbc5d93badb39d54f6ec8e0a5
c1ccccc1
Cl-[CH2;D2;+0:1]-[C:2]-[#16:3].[O;D1;H0:4]=[C:5](-[O;D1;H1:6])-[c:7]:[c:8](-[OH;D1;+0:9]):[c:10]>>[#16:3]-[C:2]-[CH2;D2;+0:1]-[O;H0;D2;+0:9]-[c:8](:[c:10]):[c:7]-[C:5](=[O;D1;H0:4])-[O;D1;H1:6]
57
[{"value": 57.0, "product": "NC1=CC(=C(C(=O)O)C=C1Cl)OCCSC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 56.5, "product": "NC1=CC(=C(C(=O)O)C=C1Cl)OCCSC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
25
CELSIUS
15
MINUTE
A cooled (5° C.) suspension of 60% sodium hydride oil dispersion (0.52 g, 13 mmoles) in anhydrous dimethylformamide (15 mL) under nitrogen was treated in portions with 4-amino-5-chloro-2-hydroxybenzoic acid (0.94 g, 5 mmoles), stirred for 15 minutes at 25° C., treated with (2-chloroethyl)methyl sulfide (1.66 g, 15 mmol...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic alcohol
Ether
null
null
c1ccccc1
HCl
CN(C=O)C
25
0.25
CSCCCl.Nc1cc(O)c(C(=O)O)cc1Cl>CN(C=O)C>CSCCOc1cc(N)c(Cl)cc1C(=O)O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-40169b770c9f42239cde7e0d4cb368b9
COc1cc(N)c(Cl)cc1C(=O)O.NCC12CCCN(CC1)C2>>COc1cc(N)c(Cl)cc1C(=O)NCC12CCCN(CC1)C2
NC1=CC(=C(C(=O)O)C=C1Cl)OC.C(=O)(N1C=NC=C1)N1C=NC=C1.N12CCCC(CC1)(C2)CN>>NC1=CC(=C(C(=O)NCC23CCCN(CC2)C3)C=C1Cl)OC
O[C:11]([c:10]1[c:3]([O:2][CH3:1])[cH:4][c:5]([NH2:6])[c:7]([Cl:8])[cH:9]1)=[O:12].[NH2:13][CH2:14][C:15]12[CH2:16][CH2:17][CH2:18][N:19]([CH2:20][CH2:21]1)[CH2:22]2>>[CH3:1][O:2][c:3]1[cH:4][c:5]([NH2:6])[c:7]([Cl:8])[cH:9][c:10]1[C:11](=[O:12])[NH:13][CH2:14][C:15]12[CH2:16][CH2:17][CH2:18][N:19]([CH2:20][CH2:21]1)[C...
COc1cc(N)c(Cl)cc1C(=O)O.NCC12CCCN(CC1)C2
COc1cc(N)c(Cl)cc1C(=O)NCC12CCCN(CC1)C2
null
null
O1CCCC1
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(NCC12CCCN(CC1)C2)c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C:6]-[C:7]-[NH2;D1;+0:8]>>[C:6]-[C:7]-[NH;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
70
[{"value": 70.0, "product": "NC1=CC(=C(C(=O)NCC23CCCN(CC2)C3)C=C1Cl)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 69.8, "product": "NC1=CC(=C(C(=O)NCC23CCCN(CC2)C3)C=C1Cl)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
A suspension of 4-amino-5-chloro-2-methoxybenzoic acid (1.72 g, 8.5 mmol) in anhydrous tetrahydrofuan (10 mL) under nitrogen was treated with 1,1'-carbonyldiimidazole (1.46 g, 9.0 mmol), stirred for one hour, then degassed under a stream of nitrogen for 10 minutes. A solution of 1-azabicyclo[3.2.1]octane-5-methanamine ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.C1CC2CCN(C1)C2
HO-
O1CCCC1
null
1
COc1cc(N)c(Cl)cc1C(=O)O.NCC12CCCN(CC1)C2>O1CCCC1>COc1cc(N)c(Cl)cc1C(=O)NCC12CCCN(CC1)C2
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-2a7ae11fb7f447428407b154948c0592
CNc1cc(OC)c(C(=O)O)cc1Cl.NCC12CCCN(CCC1)C2>>CNc1cc(OC)c(C(=O)NCC23CCCN(CCC2)C3)cc1Cl
N12CCCC(CCC1)(C2)CN.ClC=1C(=CC(=C(C(=O)O)C1)OC)NC.C(=O)(N1C=NC=C1)N1C=NC=C1>>N12CCCC(CCC1)(C2)CNC(C2=C(C=C(C(=C2)Cl)NC)OC)=O
O[C:9]([c:8]1[c:5]([O:6][CH3:7])[cH:4][c:3]([NH:2][CH3:1])[c:23]([Cl:24])[cH:22]1)=[O:10].[NH2:11][CH2:12][C:13]12[CH2:14][CH2:15][CH2:16][N:17]([CH2:18][CH2:19][CH2:20]1)[CH2:21]2>>[CH3:1][NH:2][c:3]1[cH:4][c:5]([O:6][CH3:7])[c:8]([C:9](=[O:10])[NH:11][CH2:12][C:13]23[CH2:14][CH2:15][CH2:16][N:17]([CH2:18][CH2:19][CH2...
CNc1cc(OC)c(C(=O)O)cc1Cl.NCC12CCCN(CCC1)C2
CNc1cc(OC)c(C(=O)NCC23CCCN(CCC2)C3)cc1Cl
null
null
CO.O1CCCC1
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(NCC12CCCN(CCC1)C2)c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C:6]-[C:7]-[NH2;D1;+0:8]>>[C:6]-[C:7]-[NH;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
73.3
[{"value": 73.0, "product": "N12CCCC(CCC1)(C2)CNC(C2=C(C=C(C(=C2)Cl)NC)OC)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 73.3, "product": "N12CCCC(CCC1)(C2)CNC(C2=C(C=C(C(=C2)Cl)NC)OC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
1
HOUR
A solution of 5-chloro-2-methoxy-4-(methylamino)benzoic acid (1.08 g, 5 mmol) in anhydrous tetrahydrofuran (7 mL) under nitrogen was treated with 1,1'-carbonyldiimidazole (0.90 g, 5.5 mmol), stirred one hour, degassed under a stream of nitrogen for 10 minutes, and cooled (0° C.). A solution of 1-azabicyclo[3.3.1]nonane...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.C1CC2CCCN(C1)C2
HO-
CO.O1CCCC1
0
1
CNc1cc(OC)c(C(=O)O)cc1Cl.NCC12CCCN(CCC1)C2>CO.O1CCCC1>CNc1cc(OC)c(C(=O)NCC23CCCN(CCC2)C3)cc1Cl
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-27b03df9a5db4ae9b9cafbfe76f1aac5
COCCOc1cc(N)c(Cl)cc1C(=O)O.NCC12CCCN(CCC1)C2>>COCCOc1cc(N)c(Cl)cc1C(=O)NCC12CCCN(CCC1)C2
N12CCCC(CCC1)(C2)CN.NC1=CC(=C(C(=O)O)C=C1Cl)OCCOC.C(=O)(N1C=NC=C1)N1C=NC=C1>>NC1=CC(=C(C(=O)NCC23CCCN(CCC2)C3)C=C1Cl)OCCOC
O[C:14]([c:13]1[c:6]([O:5][CH2:4][CH2:3][O:2][CH3:1])[cH:7][c:8]([NH2:9])[c:10]([Cl:11])[cH:12]1)=[O:15].[NH2:16][CH2:17][C:18]12[CH2:19][CH2:20][CH2:21][N:22]([CH2:23][CH2:24][CH2:25]1)[CH2:26]2>>[CH3:1][O:2][CH2:3][CH2:4][O:5][c:6]1[cH:7][c:8]([NH2:9])[c:10]([Cl:11])[cH:12][c:13]1[C:14](=[O:15])[NH:16][CH2:17][C:18]1...
COCCOc1cc(N)c(Cl)cc1C(=O)O.NCC12CCCN(CCC1)C2
COCCOc1cc(N)c(Cl)cc1C(=O)NCC12CCCN(CCC1)C2
null
null
O1CCCC1
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(NCC12CCCN(CCC1)C2)c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C:6]-[C:7]-[NH2;D1;+0:8]>>[C:6]-[C:7]-[NH;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
49
[{"value": 49.0, "product": "NC1=CC(=C(C(=O)NCC23CCCN(CCC2)C3)C=C1Cl)OCCOC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 49.0, "product": "NC1=CC(=C(C(=O)NCC23CCCN(CCC2)C3)C=C1Cl)OCCOC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
1
HOUR
A solution of 4-amino-5-chloro-2-(2-methoxyethoxy)benzoic acid (2.09 g, 8.5 mmol) in anhydrous tetrahydrofuran (10 mL) under nitrogen was treated with 1,1'-carbonyldiimidazole (1.46 g, 9.0 mmol), stirred for one hour, degassed under a stream of nitrogen over 10 minutes, and cooled (0° C.). A solution of 1-azabicyclo[3....
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.C1CC2CCCN(C1)C2
HO-
O1CCCC1
0
1
COCCOc1cc(N)c(Cl)cc1C(=O)O.NCC12CCCN(CCC1)C2>O1CCCC1>COCCOc1cc(N)c(Cl)cc1C(=O)NCC12CCCN(CCC1)C2
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-29b0a5406f954cd686619309354da83b
NCC12CCCN(CCC1)C2.O=C(O)c1c[nH]c2ccccc12>>O=C(NCC12CCCN(CCC1)C2)c1c[nH]c2ccccc12
C[O-].[Na+].CO.S(=O)(Cl)Cl.N12CCCC(CCC1)(C2)CN.C(C)N(CC)CC.N1C=C(C2=CC=CC=C12)C(=O)O>>N12CCCC(CCC1)(C2)CNC(=O)C2=CNC1=CC=CC=C21
[NH2:3][CH2:4][C:5]12[CH2:6][CH2:7][CH2:8][N:9]([CH2:10][CH2:11][CH2:12]1)[CH2:13]2.O[C:2](=[O:1])[c:14]1[cH:15][nH:16][c:17]2[cH:18][cH:19][cH:20][cH:21][c:22]12>>[O:1]=[C:2]([NH:3][CH2:4][C:5]12[CH2:6][CH2:7][CH2:8][N:9]([CH2:10][CH2:11][CH2:12]1)[CH2:13]2)[c:14]1[cH:15][nH:16][c:17]2[cH:18][cH:19][cH:20][cH:21][c:22...
NCC12CCCN(CCC1)C2.O=C(O)c1c[nH]c2ccccc12
O=C(NCC12CCCN(CCC1)C2)c1c[nH]c2ccccc12
null
null
O1CCCC1
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(NCC12CCCN(CCC1)C2)c1c[nH]c2ccccc12
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5]:[c:6]:[c:7]:1.[C:8]-[C:9]-[NH2;D1;+0:10]>>[C:8]-[C:9]-[NH;D2;+0:10]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5]:[c:6]:[c:7]:1
57.2
[{"value": 57.0, "product": "N12CCCC(CCC1)(C2)CNC(=O)C2=CNC1=CC=CC=C21", "details": "PERCENTYIELD", "is_desired": false}, {"value": 57.2, "product": "N12CCCC(CCC1)(C2)CNC(=O)C2=CNC1=CC=CC=C21", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
55
CELSIUS
1
HOUR
A cooled (0° C.) suspension/solution of indole-3-carboxylic acid (0.92 g, 5.7 mmol) in anhydrous tetrahydrofuran (10 mL) was treated dropwise with thionyl chloride (0.72 g, 6.0 mmol), and the solution was refluxed for one hour and concentrated in vacuo. A cooled (0° C.) solution of 1-azabicyclo[3.3.1]nonane-5-methanami...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
C1CC2CCCN(C1)C2.c1ccc2[nH]ccc2c1
HO-
O1CCCC1
55
1
NCC12CCCN(CCC1)C2.O=C(O)c1c[nH]c2ccccc12>O1CCCC1>O=C(NCC12CCCN(CCC1)C2)c1c[nH]c2ccccc12
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-5e3856e4880a45e59753efe824ac617e
Cn1cc(C(=O)O)c2ccccc21.NCC12CCCN(CCC1)C2>>O=C(NCC12CCCN(CCC1)C2)c1c[nH]c2ccccc12
N12CCCC(CCC1)(C2)CN.CN1C=C(C2=CC=CC=C12)C(=O)O.C(=O)(N1C=NC=C1)N1C=NC=C1.CN(C=O)C>>N12CCCC(CCC1)(C2)CNC(=O)C2=CNC1=CC=CC=C21
C[n:16]1[cH:15][c:14]([C:2](O)=[O:1])[c:22]2[c:17]1[cH:18][cH:19][cH:20][cH:21]2.[NH2:3][CH2:4][C:5]12[CH2:6][CH2:7][CH2:8][N:9]([CH2:10][CH2:11][CH2:12]1)[CH2:13]2>>[O:1]=[C:2]([NH:3][CH2:4][C:5]12[CH2:6][CH2:7][CH2:8][N:9]([CH2:10][CH2:11][CH2:12]1)[CH2:13]2)[c:14]1[cH:15][nH:16][c:17]2[cH:18][cH:19][cH:20][cH:21][c:...
Cn1cc(C(=O)O)c2ccccc21.NCC12CCCN(CCC1)C2
O=C(NCC12CCCN(CCC1)C2)c1c[nH]c2ccccc12
null
null
CO.C(Cl)Cl.O1CCCC1
Acylation
OtherReaction
bc16af2d4a965c15729fe77d296d53d42b81335eb8cb47aa1eea0c3f040c41cc
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(NCC12CCCN(CCC1)C2)c1c[nH]c2ccccc12
C-[n;H0;D3;+0:1]1:[c:2]:[c:3](-[C;H0;D3;+0:4](-O)=[O;D1;H0:5]):[c:6]:[c:7]:1:[c:8].[C:9]-[C:10]-[NH2;D1;+0:11]>>[C:9]-[C:10]-[NH;D2;+0:11]-[C;H0;D3;+0:4](=[O;D1;H0:5])-[c:3]1:[c:2]:[nH;D2;+0:1]:[c:7](:[c:8]):[c:6]:1
79.6
[{"value": 76.0, "product": "N12CCCC(CCC1)(C2)CNC(=O)C2=CNC1=CC=CC=C21", "details": "PERCENTYIELD", "is_desired": false}, {"value": 79.6, "product": "N12CCCC(CCC1)(C2)CNC(=O)C2=CNC1=CC=CC=C21", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
10
MINUTE
A solution of 1-methyl-1H-indole-3-carboxylic acid (1.53 g, 8.7 mmol) in anhydrous tetrahydrofuran (8 mL) under nitrogen was treated with 1.49 g (9.2 mmol) of 1,1'-carbonyldiimidazole (CDI) and stirred for 10 minutes. At this point a thick suspension formed, and anhydrous N,N-dimethylformamide (8 mL) was added. After a...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
c1c[nH]c2ccccc12
c1ccc2[nH]ccc2c1
C1CC2CCCN(C1)C2.c1ccc2[nH]ccc2c1
HO-
CO.C(Cl)Cl.O1CCCC1
null
0.166667
Cn1cc(C(=O)O)c2ccccc21.NCC12CCCN(CCC1)C2>CO.C(Cl)Cl.O1CCCC1>O=C(NCC12CCCN(CCC1)C2)c1c[nH]c2ccccc12
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-249065f6497c4fd0a7b024f92416e2ba
COc1cc(N)c(Cl)cc1C(=O)O.OCC12CCCN(CC1)C2>>COc1cc(N)c(Cl)cc1C(=O)OCC12CCCN(CC1)C2
C(CCC)[Li].CCCCCC.N12CCCC(CC1)(C2)CO.NC1=CC(=C(C(=O)O)C=C1Cl)OC.C(=O)(N1C=NC=C1)N1C=NC=C1>>N12CCCC(CC1)(C2)COC(C2=C(C=C(C(=C2)Cl)N)OC)=O
O[C:11]([c:10]1[c:3]([O:2][CH3:1])[cH:4][c:5]([NH2:6])[c:7]([Cl:8])[cH:9]1)=[O:12].[OH:13][CH2:14][C:15]12[CH2:16][CH2:17][CH2:18][N:19]([CH2:20][CH2:21]1)[CH2:22]2>>[CH3:1][O:2][c:3]1[cH:4][c:5]([NH2:6])[c:7]([Cl:8])[cH:9][c:10]1[C:11](=[O:12])[O:13][CH2:14][C:15]12[CH2:16][CH2:17][CH2:18][N:19]([CH2:20][CH2:21]1)[CH2...
COc1cc(N)c(Cl)cc1C(=O)O.OCC12CCCN(CC1)C2
COc1cc(N)c(Cl)cc1C(=O)OCC12CCCN(CC1)C2
null
null
O1CCCC1
Protection
Esterification of Carboxylic Acids
070670f68a20c1021da94fabee54def4688122fb721af5f52cd5a03630845d0e
0d8a72b7375d91aa7263e766e03a3cb7c4fa91e27abcd590409ff03b98eed690
O=C(OCC12CCCN(CC1)C2)c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C:6]-[C:7]-[OH;D1;+0:8]>>[C:6]-[C:7]-[O;H0;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
47.3
[{"value": 47.0, "product": "N12CCCC(CC1)(C2)COC(C2=C(C=C(C(=C2)Cl)N)OC)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 47.3, "product": "N12CCCC(CC1)(C2)COC(C2=C(C=C(C(=C2)Cl)N)OC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
A solution of 4-amino-5-chloro-2-methoxybenzoic acid (1.62 g, 8.0 mmol) in anhydrous tetrahydrofuran (10 mL) under nitrogen was treated with 1,1'-carbonyldiimidazole (1.38 g, 8.5 mmol), stirred one hour, and degassed under a stream of nitrogen over 10 minutes. Meanwhile, a cooled (-10° C.) solution of 1-azabicyclo[3.2....
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary alcohol
Ester
null
null
c1ccccc1.C1CC2CCN(C1)C2
HO-
O1CCCC1
null
1
COc1cc(N)c(Cl)cc1C(=O)O.OCC12CCCN(CC1)C2>O1CCCC1>COc1cc(N)c(Cl)cc1C(=O)OCC12CCCN(CC1)C2
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-6541df2d7c0d4d2fa50faf847fad032f
O=C(O)c1c[nH]c2ccccc12.OCC12CCCN(CC1)C2>>O=C(OCC12CCCN(CC1)C2)c1c[nH]c2ccccc12
C(CCC)[Li].CCCCCC.N12CCCC(CC1)(C2)CO.N1C=C(C2=CC=CC=C12)C(=O)O.C(=O)(N1C=NC=C1)N1C=NC=C1>>N12CCCC(CC1)(C2)COC(=O)C2=CNC1=CC=CC=C21
O[C:2](=[O:1])[c:13]1[cH:14][nH:15][c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]12.[OH:3][CH2:4][C:5]12[CH2:6][CH2:7][CH2:8][N:9]([CH2:10][CH2:11]1)[CH2:12]2>>[O:1]=[C:2]([O:3][CH2:4][C:5]12[CH2:6][CH2:7][CH2:8][N:9]([CH2:10][CH2:11]1)[CH2:12]2)[c:13]1[cH:14][nH:15][c:16]2[cH:17][cH:18][cH:19][cH:20][c:21]12
O=C(O)c1c[nH]c2ccccc12.OCC12CCCN(CC1)C2
O=C(OCC12CCCN(CC1)C2)c1c[nH]c2ccccc12
null
null
O1CCCC1
Protection
Esterification of Carboxylic Acids
070670f68a20c1021da94fabee54def4688122fb721af5f52cd5a03630845d0e
0d8a72b7375d91aa7263e766e03a3cb7c4fa91e27abcd590409ff03b98eed690
O=C(OCC12CCCN(CC1)C2)c1c[nH]c2ccccc12
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5]:[c:6]:[c:7]:1.[C:8]-[C:9]-[OH;D1;+0:10]>>[C:8]-[C:9]-[O;H0;D2;+0:10]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5]:[c:6]:[c:7]:1
52.4
[{"value": 52.0, "product": "N12CCCC(CC1)(C2)COC(=O)C2=CNC1=CC=CC=C21", "details": "PERCENTYIELD", "is_desired": false}, {"value": 52.4, "product": "N12CCCC(CC1)(C2)COC(=O)C2=CNC1=CC=CC=C21", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
A solution of indole-3-carboxylic acid (1.45 g, 9 mmol) in anhydrous tetrahydrofuran (10 mL) under nitrogen was treated with 1,1'-carbonyldiimidazole (1.53 g, 9.4 mmol), stirred for one hour, and degassed with a stream of nitrogen over 10 minutes. Meanwhile, a cooled (-10° C.) solution of 1-azabicyclo[3.2.1]octane-5-me...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary alcohol
Ester
null
null
C1CC2CCN(C1)C2.c1ccc2[nH]ccc2c1
HO-
O1CCCC1
null
1
O=C(O)c1c[nH]c2ccccc12.OCC12CCCN(CC1)C2>O1CCCC1>O=C(OCC12CCCN(CC1)C2)c1c[nH]c2ccccc12
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-a25b2cb2221d43fab68ec429840ec1e6
Cn1cc(C(=O)O)c2ccccc21.OCC12CCCN(CC1)C2>>Cn1cc(C(=O)OCC23CCCN(CC2)C3)c2ccccc21
C(CCC)[Li].CCCCCC.N12CCCC(CC1)(C2)CO.CN1C=C(C2=CC=CC=C12)C(=O)O.C(=O)(N1C=NC=C1)N1C=NC=C1>>N12CCCC(CC1)(C2)COC(=O)C2=CN(C1=CC=CC=C21)C
O[C:5]([c:4]1[cH:3][n:2]([CH3:1])[c:22]2[c:17]1[cH:18][cH:19][cH:20][cH:21]2)=[O:6].[OH:7][CH2:8][C:9]12[CH2:10][CH2:11][CH2:12][N:13]([CH2:14][CH2:15]1)[CH2:16]2>>[CH3:1][n:2]1[cH:3][c:4]([C:5](=[O:6])[O:7][CH2:8][C:9]23[CH2:10][CH2:11][CH2:12][N:13]([CH2:14][CH2:15]2)[CH2:16]3)[c:17]2[cH:18][cH:19][cH:20][cH:21][c:22...
Cn1cc(C(=O)O)c2ccccc21.OCC12CCCN(CC1)C2
Cn1cc(C(=O)OCC23CCCN(CC2)C3)c2ccccc21
null
null
O1CCCC1
Acylation
Esterification of Carboxylic Acids
d9bd78214ee7dbc907e499722ae01849a72d188753963443e5df9fe42c31c43b
3652e761944e8ef7ee40675a156c8ae39909c72166786934d88652debf2ec1ac
O=C(OCC12CCCN(CC1)C2)c1c[nH]c2ccccc12
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[c:5]:[#7;a:6](-[C;D1;H3:7]):[c:8]:1.[C:9]-[C:10]-[OH;D1;+0:11]>>[C:9]-[C:10]-[O;H0;D2;+0:11]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[c:5]:[#7;a:6](-[C;D1;H3:7]):[c:8]:1
58
[{"value": 58.0, "product": "N12CCCC(CC1)(C2)COC(=O)C2=CN(C1=CC=CC=C21)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 57.6, "product": "N12CCCC(CC1)(C2)COC(=O)C2=CN(C1=CC=CC=C21)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
A solution of 1-methyl-1H-indole-3-carboxylic acid (1.75 g, 10 mmol) in anhydrous tetrahydrofuran (10 mL) under nitrogen was treated with 1,1'-carbonyldiimidazole (1.79 g, 11 mmol), stirred for one hour, and degassed under a stream of nitrogen over 10 minutes. Meanwhile a cooled (-10° C.) solution of 1-azabicyclo[3.2.1...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary alcohol
Ester
null
null
C1CC2CCN(C1)C2.c1c[nH]c2ccccc12
HO-
O1CCCC1
null
1
Cn1cc(C(=O)O)c2ccccc21.OCC12CCCN(CC1)C2>O1CCCC1>Cn1cc(C(=O)OCC23CCCN(CC2)C3)c2ccccc21
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-9f608317b9754efda2c9e04eca249eb4
COc1cc(N)c(Cl)cc1C(=O)O.OCC12CCCN(CCC1)C2>>COc1cc(N)c(Cl)cc1C(=O)OCC12CCCN(CCC1)C2
C(CCC)[Li].CCCCCC.N12CCCC(CCC1)(C2)CO.NC1=CC(=C(C(=O)O)C=C1Cl)OC.C(=O)(N1C=NC=C1)N1C=NC=C1>>N12CCCC(CCC1)(C2)COC(C2=C(C=C(C(=C2)Cl)N)OC)=O
O[C:11]([c:10]1[c:3]([O:2][CH3:1])[cH:4][c:5]([NH2:6])[c:7]([Cl:8])[cH:9]1)=[O:12].[OH:13][CH2:14][C:15]12[CH2:16][CH2:17][CH2:18][N:19]([CH2:20][CH2:21][CH2:22]1)[CH2:23]2>>[CH3:1][O:2][c:3]1[cH:4][c:5]([NH2:6])[c:7]([Cl:8])[cH:9][c:10]1[C:11](=[O:12])[O:13][CH2:14][C:15]12[CH2:16][CH2:17][CH2:18][N:19]([CH2:20][CH2:2...
COc1cc(N)c(Cl)cc1C(=O)O.OCC12CCCN(CCC1)C2
COc1cc(N)c(Cl)cc1C(=O)OCC12CCCN(CCC1)C2
null
null
O1CCCC1
Protection
Esterification of Carboxylic Acids
070670f68a20c1021da94fabee54def4688122fb721af5f52cd5a03630845d0e
0d8a72b7375d91aa7263e766e03a3cb7c4fa91e27abcd590409ff03b98eed690
O=C(OCC12CCCN(CCC1)C2)c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C:6]-[C:7]-[OH;D1;+0:8]>>[C:6]-[C:7]-[O;H0;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
57.3
[{"value": 57.0, "product": "N12CCCC(CCC1)(C2)COC(C2=C(C=C(C(=C2)Cl)N)OC)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 57.3, "product": "N12CCCC(CCC1)(C2)COC(C2=C(C=C(C(=C2)Cl)N)OC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
A solution of 4-amino-5-chloro-2-methoxybenzoic acid (2.02 g, 10 mmol) in anhydrous tetrahydrofuran (10 mL) under nitrogen was treated with 1,1'-carbonyldiimidazole (1.70 g, 10.5 mmol), stirred for one hour, then degassed with a stream of nitrogen over 10 minutes. Meanwhile, a cooled (-10° C.) solution of 1-azabicyclo[...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary alcohol
Ester
null
null
c1ccccc1.C1CC2CCCN(C1)C2
HO-
O1CCCC1
null
1
COc1cc(N)c(Cl)cc1C(=O)O.OCC12CCCN(CCC1)C2>O1CCCC1>COc1cc(N)c(Cl)cc1C(=O)OCC12CCCN(CCC1)C2
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-805756e25c6e47c98a7e9f3b4a6eca54
O=C(O)c1c[nH]c2ccccc12.OCC12CCCN(CCC1)C2>>O=C(OCC12CCCN(CCC1)C2)c1c[nH]c2ccccc12
C(CCC)[Li].CCCCCC.N12CCCC(CCC1)(C2)CO.N1C=C(C2=CC=CC=C12)C(=O)O.C(=O)(N1C=NC=C1)N1C=NC=C1>>N12CCCC(CCC1)(C2)COC(=O)C2=CNC1=CC=CC=C21
O[C:2](=[O:1])[c:14]1[cH:15][nH:16][c:17]2[cH:18][cH:19][cH:20][cH:21][c:22]12.[OH:3][CH2:4][C:5]12[CH2:6][CH2:7][CH2:8][N:9]([CH2:10][CH2:11][CH2:12]1)[CH2:13]2>>[O:1]=[C:2]([O:3][CH2:4][C:5]12[CH2:6][CH2:7][CH2:8][N:9]([CH2:10][CH2:11][CH2:12]1)[CH2:13]2)[c:14]1[cH:15][nH:16][c:17]2[cH:18][cH:19][cH:20][cH:21][c:22]1...
O=C(O)c1c[nH]c2ccccc12.OCC12CCCN(CCC1)C2
O=C(OCC12CCCN(CCC1)C2)c1c[nH]c2ccccc12
null
null
O1CCCC1
Protection
Esterification of Carboxylic Acids
070670f68a20c1021da94fabee54def4688122fb721af5f52cd5a03630845d0e
0d8a72b7375d91aa7263e766e03a3cb7c4fa91e27abcd590409ff03b98eed690
O=C(OCC12CCCN(CCC1)C2)c1c[nH]c2ccccc12
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5]:[c:6]:[c:7]:1.[C:8]-[C:9]-[OH;D1;+0:10]>>[C:8]-[C:9]-[O;H0;D2;+0:10]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3]1:[c:4]:[#7;a:5]:[c:6]:[c:7]:1
60
[{"value": 60.0, "product": "N12CCCC(CCC1)(C2)COC(=O)C2=CNC1=CC=CC=C21", "details": "PERCENTYIELD", "is_desired": false}, {"value": 60.0, "product": "N12CCCC(CCC1)(C2)COC(=O)C2=CNC1=CC=CC=C21", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
A solution of indole-3-carboxylic acid (1.62 g, 10 mmol) in anhydrous tetrahydrofuran (10 mL) under nitrogen was treated with 1,1'-carbonyldiimidazole (1.70 g, 10.5 mmol), stirred for one hour, and degassed with a stream of nitrogen for 10 minutes giving a suspension. Meanwhile, a cooled (-10° C.) solution of 1-azabicy...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary alcohol
Ester
null
null
C1CC2CCCN(C1)C2.c1ccc2[nH]ccc2c1
HO-
O1CCCC1
null
1
O=C(O)c1c[nH]c2ccccc12.OCC12CCCN(CCC1)C2>O1CCCC1>O=C(OCC12CCCN(CCC1)C2)c1c[nH]c2ccccc12
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-4406e0402c004a7288caf0b804f30d30
Cn1nc(C(=O)N2C=CNC2)c2ccccc21.OCC12CCCN(CC1)C2>>Cn1nc(C(=O)OCC23CCCN(CC2)C3)c2ccccc21
N12CCCC(CC1)(C2)CO.C(CCC)[Li].CCCCCC.N1(CNC=C1)C(=O)C1=NN(C2=CC=CC=C12)C>>N12CCCC(CC1)(C2)COC(=O)C2=NN(C1=CC=CC=C21)C
C1=CN([C:5]([c:4]2[n:3][n:2]([CH3:1])[c:22]3[c:17]2[cH:18][cH:19][cH:20][cH:21]3)=[O:6])CN1.[OH:7][CH2:8][C:9]12[CH2:10][CH2:11][CH2:12][N:13]([CH2:14][CH2:15]1)[CH2:16]2>>[CH3:1][n:2]1[n:3][c:4]([C:5](=[O:6])[O:7][CH2:8][C:9]23[CH2:10][CH2:11][CH2:12][N:13]([CH2:14][CH2:15]2)[CH2:16]3)[c:17]2[cH:18][cH:19][cH:20][cH:2...
Cn1nc(C(=O)N2C=CNC2)c2ccccc21.OCC12CCCN(CC1)C2
Cn1nc(C(=O)OCC23CCCN(CC2)C3)c2ccccc21
null
null
O1CCCC1
Acylation
OtherReaction
8edc29c6893178a6858d8b5ac545e0fdd2b118e1fbf01c3899745cd412374b17
0b63fdab604c55d4e8e6de999528c93d919889391aba78782e3e6672485adf50
O=C(OCC12CCCN(CC1)C2)c1n[nH]c2ccccc12
[C;D1;H3:1]-[#7;a:2]1:[#7;a:3]:[c:4](-[C;H0;D3;+0:5](=[O;D1;H0:6])-N2-C-N-C=C-2):[c:7]:[c:8]:1.[C:9]-[C:10]-[OH;D1;+0:11]>>[C:9]-[C:10]-[O;H0;D2;+0:11]-[C;H0;D3;+0:5](=[O;D1;H0:6])-[c:4]1:[#7;a:3]:[#7;a:2](-[C;D1;H3:1]):[c:8]:[c:7]:1
53.1
[{"value": 53.0, "product": "N12CCCC(CC1)(C2)COC(=O)C2=NN(C1=CC=CC=C21)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 53.1, "product": "N12CCCC(CC1)(C2)COC(=O)C2=NN(C1=CC=CC=C21)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
A cooled (0° C.) solution of 1-azabicyclo[3.2.1]oct-5-ylmethanol (1.70 g, 12 mmol) in anhydrous tetrahydrofuran (15 mL) under nitrogen was treated (via syringe) with 2.45N n-butyllithium/hexane (12 mmol), then stirred at room temperature for thirty minutes and concentrated in vacuo to remove all hexane. Anhydrous tetra...
10.6084/m9.figshare.5104873.v1
null
Enamine.Enamine.Tertiary amide.Primary alcohol
Ester
C1=CNCN1
null
C1CC2CCN(C1)C2.c1n[nH]c2ccccc12
Other
O1CCCC1
null
3
Cn1nc(C(=O)N2C=CNC2)c2ccccc21.OCC12CCCN(CC1)C2>O1CCCC1>Cn1nc(C(=O)OCC23CCCN(CC2)C3)c2ccccc21
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-1339d8a661144dc8b56716544887dca6
C=CCOc1cc(N)c(Cl)cc1C(=O)O.NCC12CCCN(CC1)C2>>C=CCOc1cc(N)c(Cl)cc1C(=O)NCC12CCCN(CC1)C2
NC1=CC(=C(C(=O)O)C=C1Cl)OCC=C.N12CCCC(CC1)(C2)CN>>NC1=CC(=C(C(=O)NCC23CCCN(CC2)C3)C=C1Cl)OCC=C
O[C:13]([c:12]1[c:5]([O:4][CH2:3][CH:2]=[CH2:1])[cH:6][c:7]([NH2:8])[c:9]([Cl:10])[cH:11]1)=[O:14].[NH2:15][CH2:16][C:17]12[CH2:18][CH2:19][CH2:20][N:21]([CH2:22][CH2:23]1)[CH2:24]2>>[CH2:1]=[CH:2][CH2:3][O:4][c:5]1[cH:6][c:7]([NH2:8])[c:9]([Cl:10])[cH:11][c:12]1[C:13](=[O:14])[NH:15][CH2:16][C:17]12[CH2:18][CH2:19][CH...
C=CCOc1cc(N)c(Cl)cc1C(=O)O.NCC12CCCN(CC1)C2
C=CCOc1cc(N)c(Cl)cc1C(=O)NCC12CCCN(CC1)C2
null
null
null
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C(NCC12CCCN(CC1)C2)c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[C:6]-[C:7]-[NH2;D1;+0:8]>>[C:6]-[C:7]-[NH;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
null
[]
null
null
null
null
Following the procedure of Example 1, the title compound is prepared from 4-amino-5-chloro-2-(2-propenyloxy)benzoic acid and 1-azabicyclo[3.2.1]octan-5-methanamine. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
c1ccccc1.C1CC2CCN(C1)C2
HO-
null
null
null
C=CCOc1cc(N)c(Cl)cc1C(=O)O.NCC12CCCN(CC1)C2>>C=CCOc1cc(N)c(Cl)cc1C(=O)NCC12CCCN(CC1)C2
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-e3905ec671db4476912df221b80d4a05
CCOC(=O)C=[N+]=[N-].O=C1CCCCCCC1>>CCOC(=O)C1CCCCCCCC1=O
C1(CCCCCCC1)=O.F[B-](F)(F)F.C(C)[O+](CC)CC.[N+](=[N-])=CC(=O)OCC>>C(C)OC(=O)C1C(CCCCCCC1)=O
[N-]=[N+]=[CH:6][C:4]([O:3][CH2:2][CH3:1])=[O:5].[CH2:7]1[CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][CH2:13][C:14]1=[O:15]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]1[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][CH2:13][C:14]1=[O:15]
CCOC(=O)C=[N+]=[N-].O=C1CCCCCCC1
CCOC(=O)C1CCCCCCCC1=O
null
null
C(Cl)Cl
C-C Coupling
OtherReaction
f4358bd2f3aee366b34c2d0a955f09f77d20286ffd3a4c0291e733957f7927ad
4f5428734ef204d1fb311ee2d76e19b4e3b64154d65d22fa6a8abd7ae101915a
O=C1CCCCCCCC1
[C:1]-[#8:2]-[C:3](=[O;D1;H0:4])-[CH;D2;+0:5]=[N+]=[N-].[C:6]-[C:7]-[C;H0;D3;+0:8](=[O;D1;H0:9])-[CH2;D2;+0:10]-[C:11]-[C:12]>>[C:6]-[C:7]-[C;H0;D3;+0:8](=[O;D1;H0:9])-[CH;D3;+0:5](-[C:3](=[O;D1;H0:4])-[#8:2]-[C:1])-[CH2;D2;+0:10]-[C:11]-[C:12]
null
[]
0
CELSIUS
4
HOUR
Cyclooctanone (25 g, 198 mmol) is dissolved in methylene chloride (500 mL) and the solution is cooled to 0° C. Triethyloxonium tetrafluoroborate (121.6 g, 640 mmol) is added. Ethyl diazoacetate (41.61 g, 365 mmol) is then added dropwise over 25 minutes, and the reaction is stirred at 0° C. for 4 hours. The reaction is ...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ester.Diazo
Ketone.Ester
C1CCCCCCC1
C1CCCCCCCC1
C1CCCCCCCC1
Other
C(Cl)Cl
0
4
CCOC(=O)C=[N+]=[N-].O=C1CCCCCCC1>C(Cl)Cl>CCOC(=O)C1CCCCCCCC1=O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-457a83af2b8e486aa8de7028583f3486
CCOC(=O)C1CCCCCCCC1=O.[NH4+]>>CCOC(=O)C1CCCCCCCC(=O)N1
[OH-].[NH4+].CS(=O)(=O)O.C(C)OC(=O)C1C(CCCCCCC1)=O.[N-]=[N+]=[N-].[Na+]>>O=C1NC(CCCCCCC1)C(=O)OCC
[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]1[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][CH2:13][C:14]1=[O:15].[NH4+:16]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]1[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][CH2:13][C:14](=[O:15])[NH:16]1
CCOC(=O)C1CCCCCCCC1=O.[NH4+]
CCOC(=O)C1CCCCCCCC(=O)N1
null
null
C(Cl)(Cl)Cl
Functional Group Addition
OtherReaction
dab08ea5b22dba23d2341d507cac6bea4785139ff0bce40600f0aa70079110c9
579fa31aaf6029bc11db649a382a0ef8bdbfe77711c459bfaf065d9de2dbfbb7
O=C1CCCCCCCCN1
[C:1]-[C:2]-[C;H0;D3;+0:3](=[O;D1;H0:4])-[CH;D3;+0:5](-[C:6](=[O;D1;H0:7])-[#8:8]-[C:9])-[C:10]-[C:11].[NH4+;D0:12]>>[C:1]-[C:2]-[C;H0;D3;+0:3](=[O;D1;H0:4])-[NH;D2;+0:12]-[CH;D3;+0:5](-[C:6](=[O;D1;H0:7])-[#8:8]-[C:9])-[C:10]-[C:11]
null
[]
0
CELSIUS
30
MINUTE
2-Ethoxycarbonyl-cyclononanone (13.72 g, 64.7 mmol) is dissolved in chloroform (200 mL) and cooled to 0° C. Methanesulfonic acid (62.4 g, 650 mmol) is added, followed by sodium azide (12.68 g, 195 mmol). The reaction is stirred at room temperature for 30 minutes, and then heated to reflux for 4 hours. The reaction mixt...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ester
Ester.Secondary amide
C1CCCCCCCC1
C1CCCCNCCCC1
C1CCCCNCCCC1
null
C(Cl)(Cl)Cl
0
0.5
CCOC(=O)C1CCCCCCCC1=O.[NH4+]>C(Cl)(Cl)Cl>CCOC(=O)C1CCCCCCCC(=O)N1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-506b9adb631a461cb9ffccba8d2f7bb0
BrBr.CCOC(=O)C1CCCCCCCC(=O)N1>>CCOC(=O)[C@@H]1CCCCCC[C@H](Br)C(=O)N1
BrBr.P(Cl)(Cl)(Cl)(Cl)Cl.II.O=C1NC(CCCCCCC1)C(=O)OCC>>Br[C@@H]1C(N[C@@H](CCCCCC1)C(=O)OCC)=O
Br[Br:14].[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]1[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][CH2:13][C:15](=[O:16])[NH:17]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[C@@H:6]1[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][C@H:13]([Br:14])[C:15](=[O:16])[NH:17]1
BrBr.CCOC(=O)C1CCCCCCCC(=O)N1
CCOC(=O)[C@@H]1CCCCCC[C@H](Br)C(=O)N1
null
null
C(Cl)Cl
Functional Group Interconversion
Bromination
0eec1c7220b5e11cd6f23f5cad283ea61e0679382fe547aa2e4e5e76415cfb6a
0c353a1260488c22c3ffb72de5623420c3ec35470a0b3a2045b11c29224f458e
O=C1CCCCCCCCN1
Br-[Br;H0;D1;+0:1].[#8:2]-[C:3](=[O;D1;H0:4])-[C:5]-[#7:6]-[C:7](=[O;D1;H0:8])-[CH2;D2;+0:9]-[C:10]-[C:11]>>[#8:2]-[C:3](=[O;D1;H0:4])-[C:5]-[#7:6]-[C:7](=[O;D1;H0:8])-[C@@H;D3;+0:9](-[Br;H0;D1;+0:1])-[C:10]-[C:11]
null
[]
0
CELSIUS
15
MINUTE
Ethyl 2-oxo-1-azacyclodecane-10-carboxylate (4.0 g, 17.6 mmol) is dissolved in methylene chloride (50 mL), and cooled to 0° C. Phosphorus pentachloride (3.85 g, 18.5 mmol) and iodine (0.051 g, 0.2 mmol) are added. The reaction is stirred for 15 minutes at 0° C. Then, bromine (3.10 g, 19.4 mmol) is added, and the reacti...
10.6084/m9.figshare.5104873.v1
null
null
Secondary halide
C1CCCCNCCCC1
C1CCCCNCCCC1
C1CCCCNCCCC1
HBr
C(Cl)Cl
0
0.25
BrBr.CCOC(=O)C1CCCCCCCC(=O)N1>C(Cl)Cl>CCOC(=O)[C@@H]1CCCCCC[C@H](Br)C(=O)N1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-dcb68cc3bff744d997cc097884f62d34
CCOC(=O)[C@@H]1CCCCCC[C@H](Br)C(=O)N1>>CCOC(=O)[C@@H]1CCCCCC[C@H](OC(C)=O)C(=O)N1
Br[C@@H]1C(N[C@@H](CCCCCC1)C(=O)OCC)=O>>C(C)(=O)O[C@@H]1C(N[C@@H](CCCCCC1)C(=O)OCC)=O
Br[C@H:13]1[CH2:12][CH2:11][CH2:10][CH2:1][CH2:8][CH2:7][C@@H:6]([C:4](=[O:3])[O:14][CH2:15][CH3:16])[NH:20][C:18]1=[O:19]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[C@@H:6]1[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][C@H:13]([O:14][C:15]([CH3:16])=[O:17])[C:18](=[O:19])[NH:20]1
CCOC(=O)[C@@H]1CCCCCC[C@H](Br)C(=O)N1
CCOC(=O)[C@@H]1CCCCCC[C@H](OC(C)=O)C(=O)N1
null
C(C)(=O)[O-].[Ag+]
CN(C=O)C.C(C)(=O)OCC
Miscellaneous
OtherReaction
13d89ff76626018539378bea9b2dd36c53f4d944ec29433c9578ce63d5256397
6525c54fe846f0fa59c15bd6b671acee5a1b77633e0eba0e10f45d27e96ae1f5
O=C1CCCCCCCCN1
Br-[C@H;D3;+0:1]1-[C:2]-[C:3]-[CH2;D2;+0:4]-[CH2;D2;+0:5]-[CH2;D2;+0:6]-[C:7]-[C:8](-[C;H0;D3;+0:9](=[O;H0;D1;+0:10])-[O;H0;D2;+0:11]-[CH2;D2;+0:12]-[C;D1;H3:13])-[#7:14]-[C:15]-1=[O;D1;H0:16]>>[C;D1;H3:13]-[C;H0;D3;+0:12](=[O;D1;H0:17])-[O;H0;D2;+0:11]-[C@H;D3;+0:1]1-[C:2]-[C:3]-[CH2;D2;+0:4]-[C:18]-[CH2;D2;+0:6]-[C:7...
null
[]
100
CELSIUS
null
null
Cis ethyl 3-bromo-2-oxo-1-azacyclodecane-10-carboxylate (2.96 g, 9.67 mmol) is dissolved in dimethylformamide (30 mL). Silver acetate (6.35 g, 38 mmol) is added, and the reaction is heated to 100° C. for 3 hours. After cooling back to room temperature, the reaction is diluted with ethyl acetate (100 mL), filtered throu...
10.6084/m9.figshare.5104873.v1
null
Secondary halide.Ester
Ester.Ester
C1CCCCNCCCC1
C1CCCCNCCCC1
C1CCCCNCCCC1
Br-
C(C)(=O)[O-].[Ag+].CN(C=O)C.C(C)(=O)OCC
100
null
CCOC(=O)[C@@H]1CCCCCC[C@H](Br)C(=O)N1>C(C)(=O)[O-].[Ag+].CN(C=O)C.C(C)(=O)OCC>CCOC(=O)[C@@H]1CCCCCC[C@H](OC(C)=O)C(=O)N1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-d4fb9e46ad954be7a349fa818cd8a137
CCOC(=O)C1CCCCCCC(=O)C(=O)N1.C[Si](C)(C)[CH2][Mg][Cl]>>CCOC(=O)C1CCCCCCC(O)(C[Si](C)(C)C)C(=O)N1
C[Si](C)(C)C[Mg]Cl.O=C1NC(CCCCCCC1=O)C(=O)OCC>>C[Si](C)(C)CC1(C(NC(CCCCCC1)C(=O)OCC)=O)O
[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]1[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][C:13](=[O:14])[C:20](=[O:21])[NH:22]1.[Cl][Mg][CH2:15][Si:16]([CH3:17])([CH3:18])[CH3:19]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]1[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][C:13]([OH:14])([CH2:15][Si:16]([CH3:17])([CH3:18])[CH3:19])...
CCOC(=O)C1CCCCCCC(=O)C(=O)N1.C[Si](C)(C)[CH2][Mg][Cl]
CCOC(=O)C1CCCCCCC(O)(C[Si](C)(C)C)C(=O)N1
null
null
CCOCC
C-C Coupling
Grignard from ketone to alcohol
5f5e7255c18c21fef298467b179ec1f4f56424d16c6fc1d165c33612b9c843be
5854166cd4ea706bc07d74dc79eb8f4a990bc6c5eacbf0ca947d88ee86e78fdf
O=C1CCCCCCCCN1
[#8:1]-[C:2](=[O;D1;H0:3])-[C:4]-[#7:5]-[C:6](=[O;D1;H0:7])-[C;H0;D3;+0:8](=[O;H0;D1;+0:9])-[C:10]-[C:11].[C;D1;H3:12]-[#14:13](-[C;D1;H3:14])(-[C;D1;H3:15])-[CH2;D2;+0:16]-[Mg]-[Cl]>>[#8:1]-[C:2](=[O;D1;H0:3])-[C:4]-[#7:5]-[C:6](=[O;D1;H0:7])-[C;H0;D4;+0:8](-[OH;D1;+0:9])(-[CH2;D2;+0:16]-[#14:13](-[C;D1;H3:12])(-[C;D1...
null
[]
0
CELSIUS
20
MINUTE
Ethyl 2,3-di-oxo-1-azacyclodecane-10-carboxylate (5.02 g, 20.81 mmol) is dissolved in ether (50 mL), and cooled to 0° C. Trimethylsilylmethylmagnesium chloride (42.0 mL of a 1.0M solution in ether, 42.0 mmol) is added dropwise, the reaction is stirred at 0° C. for 20 minutes, and then heated to reflux overnight. The re...
10.6084/m9.figshare.5104873.v1
null
Magnesium halide.Ketone
Tertiary alcohol
C1CCCCNCCCC1
C1CCCCNCCCC1
C1CCCCNCCCC1
Mg
CCOCC
0
0.333333
CCOC(=O)C1CCCCCCC(=O)C(=O)N1.C[Si](C)(C)[CH2][Mg][Cl]>CCOCC>CCOC(=O)C1CCCCCCC(O)(C[Si](C)(C)C)C(=O)N1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-33f9adfd6f284316b20090b99cc163ce
CCOC(=O)C1CCCCCCC(O)(C[Si](C)(C)C)C(=O)N1>>C=C1CCCCCCC(C(=O)OCC)NC1=O
C[Si](C)(C)CC1(C(NC(CCCCCC1)C(=O)OCC)=O)O.B(F)(F)F.CCOCC>>C=C1C(NC(CCCCCC1)C(=O)OCC)=O
C[Si](C)(C)[CH2:1][C:2]1(O)[CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH:9]([C:10](=[O:11])[O:12][CH2:13][CH3:14])[NH:15][C:16]1=[O:17]>>[CH2:1]=[C:2]1[CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH:9]([C:10](=[O:11])[O:12][CH2:13][CH3:14])[NH:15][C:16]1=[O:17]
CCOC(=O)C1CCCCCCC(O)(C[Si](C)(C)C)C(=O)N1
C=C1CCCCCCC(C(=O)OCC)NC1=O
null
null
C(Cl)Cl
Miscellaneous
OtherReaction
08ed58de1dbc0a0a0052264d5574865af5675238cbdaadd8f99b21f9961cf196
70726fffd1247b98d91d1ce6bd15a8de9817aaf84343b50627ddafec4dfb3c6c
C=C1CCCCCCCNC1=O
C-[Si](-C)(-C)-[CH2;D2;+0:1]-[C;H0;D4;+0:2](-O)(-[C:3]-[C:4])-[C:5](=[O;D1;H0:6])-[#7:7]-[C:8]-[C:9](-[#8:10])=[O;D1;H0:11]>>[#8:10]-[C:9](=[O;D1;H0:11])-[C:8]-[#7:7]-[C:5](=[O;D1;H0:6])-[C;H0;D3;+0:2](=[CH2;D1;+0:1])-[C:3]-[C:4]
null
[]
null
null
26
HOUR
Ethyl 3-(trimethylsilylmethyl)-3-hydroxy-2-oxo-1-azacyclodecane-10-carboxylate (0.98 g, 2.98 mmol) is dissolved in methylene chloride (50 mL), and boron trifluoride etherate (1.8 mL, 15 mmol) is added. The reaction is stirred at room temperature for 26 hours. The reaction is then quenched with saturated ammonium chlori...
10.6084/m9.figshare.5104873.v1
null
Tertiary alcohol.Silyl protective group
Vinyl
C1CCCCNCCCC1
C1CCCCNCCCC1
C1CCCCNCCCC1
HO-
C(Cl)Cl
null
26
CCOC(=O)C1CCCCCCC(O)(C[Si](C)(C)C)C(=O)N1>C(Cl)Cl>C=C1CCCCCCC(C(=O)OCC)NC1=O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-0675e965fa4340e2acbd5041468c8136
CC(=O)Cl.O=C1N[C@@H](C(=O)O)CCCCCC[C@@H]1CS>>CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)O)NC1=O
SC[C@@H]1C(N[C@H](CCCCCC1)C(=O)O)=O.C(C)(=O)Cl>>C(C)(=O)SC[C@@H]1C(N[C@H](CCCCCC1)C(=O)O)=O
Cl[C:2]([CH3:1])=[O:3].[SH:4][CH2:5][C@H:6]1[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][C@H:13]([C:14](=[O:15])[OH:16])[NH:17][C:18]1=[O:19]>>[CH3:1][C:2](=[O:3])[S:4][CH2:5][C@H:6]1[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][C@H:13]([C:14](=[O:15])[OH:16])[NH:17][C:18]1=[O:19]
CC(=O)Cl.O=C1N[C@@H](C(=O)O)CCCCCC[C@@H]1CS
CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)O)NC1=O
null
null
N1=CC=CC=C1
Acylation
thioether_nucl_sub
774e8f449f87493fdbd93fdbbfef7c7bc086966dfce8806abcb487630046ef59
cf70b55890699bc889b230d5ae9783daf8be8d20d1ad4c06197ffaf659088f4e
O=C1CCCCCCCCN1
Cl-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3].[#7:4]-[C:5](=[O;D1;H0:6])-[C:7]-[C:8]-[SH;D1;+0:9]>>[#7:4]-[C:5](=[O;D1;H0:6])-[C:7]-[C:8]-[S;H0;D2;+0:9]-[C;H0;D3;+0:1](-[C;D1;H3:2])=[O;D1;H0:3]
null
[]
null
null
8
HOUR
Trans 3-mercaptomethyl-2-oxo-1-azacyclodecane-10-carboxylic acid (0.75 g, 3.06 mmol) is dissolved in pyridine (20 mL). Acetyl chloride (0.26 g, 3.37 mmol) is added, and the reaction is stirred at room temperature overnight. The reaction is quenched by cooling to 0° C., adding concentrated hydrochloric acid (20 mL), dil...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Aliphatic thiol
Carbo-thioester
null
null
C1CCCCNCCCC1
HCl
N1=CC=CC=C1
null
8
CC(=O)Cl.O=C1N[C@@H](C(=O)O)CCCCCC[C@@H]1CS>N1=CC=CC=C1>CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)O)NC1=O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-6d7f78a9e4854515844933e38954e2d1
CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)O)NC1=O>>CC(=O)SC[C@H]1CCCCCC[C@H](C(N)=O)NC1=O
C(C)(=O)SC[C@@H]1C(N[C@H](CCCCCC1)C(=O)O)=O.CN1CCOCC1.ClC(=O)OCC>>C(C)(=O)SC[C@@H]1C(N[C@H](CCCCCC1)C(=O)N)=O
O[C:14]([C@H:13]1[CH2:12][CH2:11][CH2:10][CH2:9][CH2:8][CH2:7][C@H:6]([CH2:5][S:4][C:2]([CH3:1])=[O:3])[C:18](=[O:19])[NH:17]1)=[O:16]>>[CH3:1][C:2](=[O:3])[S:4][CH2:5][C@H:6]1[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][C@H:13]([C:14]([NH2:15])=[O:16])[NH:17][C:18]1=[O:19]
CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)O)NC1=O
CC(=O)SC[C@H]1CCCCCC[C@H](C(N)=O)NC1=O
null
null
C(Cl)Cl.O1CCCC1
Functional Group Interconversion
OtherReaction
e1b1a1f71ee10336b9e90a021457b106dbfe08a22161aaad6804675a8134a46f
5d384be3554a01fd49be5eb779c3b10075a4cc9a2373eb20aaa867286d4e28a9
O=C1CCCCCCCCN1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[#7:5]-[C:6]=[O;D1;H0:7]>>[C:4]-[C:3](-[C;H0;D3;+0:1](-[N;D1;H2:8])=[O;D1;H0:2])-[#7:5]-[C:6]=[O;D1;H0:7]
null
[]
-20
CELSIUS
30
MINUTE
Trans 3-(acetylthiomethyl)-2-oxo-1-azacyclodecane-10-carboxylic acid (0.30 g, 1.05 mmol) is dissolved in tetrahydrofuran (5.0 mL). 4-Methylmorpholine (0.14 mL, 1.05 mmol) is then added, and the reaction is cooled to -20° C. Ethyl chloroformate (0.1 mL, 1.05 mmol) is then added, and the reaction is stirred at -20° C. fo...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Primary amide
null
null
C1CCCCNCCCC1
null
C(Cl)Cl.O1CCCC1
-20
0.5
CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)O)NC1=O>C(Cl)Cl.O1CCCC1>CC(=O)SC[C@H]1CCCCCC[C@H](C(N)=O)NC1=O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-b118b628f60746c29335fc3e59194550
CC(=O)SC[C@H]1CCCCCC[C@H](C(N)=O)NC1=O>>NC(=O)[C@H]1CCCCCC[C@H](CS)C(=O)N1
C(C)(=O)SC[C@@H]1C(N[C@H](CCCCCC1)C(=O)N)=O.[OH-].[Na+].Cl>>SC[C@@H]1C(N[C@H](CCCCCC1)C(=O)N)=O
CC(=O)[S:13][CH2:12][C@H:11]1[CH2:10][CH2:9][CH2:8][CH2:7][CH2:6][CH2:5][C@H:4]([C:2]([NH2:1])=[O:3])[NH:16][C:14]1=[O:15]>>[NH2:1][C:2](=[O:3])[C@H:4]1[CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][C@H:11]([CH2:12][SH:13])[C:14](=[O:15])[NH:16]1
CC(=O)SC[C@H]1CCCCCC[C@H](C(N)=O)NC1=O
NC(=O)[C@H]1CCCCCC[C@H](CS)C(=O)N1
null
null
C(C)O
Reduction
OtherReaction
7702cd666d5d9a9f1bdea3600e3b84cc62dd11d3f2cea261702317a39db4e581
18d802456fe85193570fdb3a00b25c8956a03b5a0210f708f961e42c1669d76e
O=C1CCCCCCCCN1
C-C(=O)-[S;H0;D2;+0:1]-[C:2]-[C:3]-[C:4](=[O;D1;H0:5])-[#7:6]>>[#7:6]-[C:4](=[O;D1;H0:5])-[C:3]-[C:2]-[SH;D1;+0:1]
null
[]
null
null
1
HOUR
Trans 3-(acetylthiomethyl)-2-oxo-1-azacyclodecane-10-carboxamide (0.16 g, 0.56 mmol) is dissolved in ethanol (5.0 mL). An aqueous solution of 1N sodium hydroxide (0.60 mL, 0.60 mmol) is added, and the reaction is stirred for 1 hour. The reaction is acidified with 1N hydrochloric acid to a pH of about 3, and the solvent...
10.6084/m9.figshare.5104873.v1
null
Carbo-thioester
Aliphatic thiol
null
null
C1CCCCNCCCC1
HO-
C(C)O
null
1
CC(=O)SC[C@H]1CCCCCC[C@H](C(N)=O)NC1=O>C(C)O>NC(=O)[C@H]1CCCCCC[C@H](CS)C(=O)N1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-37b24b9090dc4d9a9382a6652abf7b0e
CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)O)NC1=O.Nc1cccnc1>>CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)Nc2cccnc2)NC1=O
C(C)(=O)SC[C@@H]1C(N[C@H](CCCCCC1)C(=O)O)=O.NC=1C=NC=CC1.ON1N=NC2=C1C=CC=C2.CN1CCOCC1.Cl.CN(C)CCCN=C=NCC>>C(C)(=O)SC[C@@H]1C(N[C@H](CCCCCC1)C(=O)NC=1C=NC=CC1)=O
O[C:14]([C@H:13]1[CH2:12][CH2:11][CH2:10][CH2:9][CH2:8][CH2:7][C@H:6]([CH2:5][S:4][C:2]([CH3:1])=[O:3])[C:24](=[O:25])[NH:23]1)=[O:15].[NH2:16][c:17]1[cH:18][cH:19][cH:20][n:21][cH:22]1>>[CH3:1][C:2](=[O:3])[S:4][CH2:5][C@H:6]1[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][C@H:13]([C:14](=[O:15])[NH:16][c:17]2[cH:18][cH...
CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)O)NC1=O.Nc1cccnc1
CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)Nc2cccnc2)NC1=O
null
null
C(Cl)Cl
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C1CCCCCCC[C@H](C(=O)Nc2cccnc2)N1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[#7:5]-[C:6]=[O;D1;H0:7].[NH2;D1;+0:8]-[c:9](:[c:10]):[c:11]:[#7;a:12]:[c:13]>>[C:4]-[C:3](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:8]-[c:9](:[c:10]):[c:11]:[#7;a:12]:[c:13])-[#7:5]-[C:6]=[O;D1;H0:7]
null
[]
0
CELSIUS
8
HOUR
Trans 3-(acetylthiomethyl)-2-oxo-1-azacyclodecane-10-carboxylic acid (0.100 g, 0.35 mmol), 3-aminopyridine (0.036 g, 0.38 mmol), 1-hydroxybenzotriazole (0.047 g, 0.035 mmol), and 4-methylmorpholine (0.077 mL, 0.70 mmol) are dissolved in methylene chloride (2.5 mL), and the reaction is cooled to 0° C. To this solution i...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
C1CCCCNCCCC1.c1ccncc1
HO-
C(Cl)Cl
0
8
CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)O)NC1=O.Nc1cccnc1>C(Cl)Cl>CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)Nc2cccnc2)NC1=O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-039d993767fd48bca5979ee161469481
CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)Nc2cccnc2)NC1=O>>O=C1N[C@@H](C(=O)Nc2cccnc2)CCCCCC[C@@H]1CS
C(C)(=O)SC[C@@H]1C(N[C@H](CCCCCC1)C(=O)NC=1C=NC=CC1)=O.Cl>>Cl.SC[C@@H]1C(N[C@H](CCCCCC1)C(=O)NC=1C=NC=CC1)=O
CC(=O)[S:23][CH2:22][C@@H:21]1[C:3](=[O:2])[NH:4][C@@H:5]([C:6](=[O:7])[NH:8][c:9]2[cH:10][cH:11][cH:12][n:13][cH:14]2)[CH2:15][CH2:16][CH2:17][CH2:18][CH2:19][CH2:20]1>>[O:2]=[C:3]1[NH:4][C@@H:5]([C:6](=[O:7])[NH:8][c:9]2[cH:10][cH:11][cH:12][n:13][cH:14]2)[CH2:15][CH2:16][CH2:17][CH2:18][CH2:19][CH2:20][C@@H:21]1[CH2...
CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)Nc2cccnc2)NC1=O
O=C1N[C@@H](C(=O)Nc2cccnc2)CCCCCC[C@@H]1CS
null
null
C(C)O
Reduction
OtherReaction
7702cd666d5d9a9f1bdea3600e3b84cc62dd11d3f2cea261702317a39db4e581
18d802456fe85193570fdb3a00b25c8956a03b5a0210f708f961e42c1669d76e
O=C1CCCCCCC[C@H](C(=O)Nc2cccnc2)N1
C-C(=O)-[S;H0;D2;+0:1]-[C:2]-[C:3]-[C:4](=[O;D1;H0:5])-[#7:6]>>[#7:6]-[C:4](=[O;D1;H0:5])-[C:3]-[C:2]-[SH;D1;+0:1]
null
[]
null
null
90
MINUTE
3-{N-[[trans 3-(acetylthiomethyl)-2-oxo-1-azacyclodecan-10-yl]-carbonyl]-amino}-pyridine (0.040 g, 0.11 mmol) is dissolved in ethanol (1.0 mL). An aqueous solution of nitrogen-degasded 1N sodium hydroxide (0.33 mL, 0.33 mmol) is added, and the reaction is stirred for 90 minutes. The reaction is quenched with 1N hydroch...
10.6084/m9.figshare.5104873.v1
null
Carbo-thioester
Aliphatic thiol
null
null
C1CCCCNCCCC1.c1ccncc1
HO-
C(C)O
null
1.5
CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)Nc2cccnc2)NC1=O>C(C)O>O=C1N[C@@H](C(=O)Nc2cccnc2)CCCCCC[C@@H]1CS
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-78b42a7c2bd74f04a8c7a9f150514491
CC(=O)OCCN.CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)O)NC1=O>>CC(=O)OCCNC(=O)[C@H]1CCCCCC[C@H](CSC(C)=O)C(=O)N1
C(C)(=O)SC[C@@H]1C(N[C@H](CCCCCC1)C(=O)O)=O.Cl.C(C)(=O)OCCN.ON1N=NC2=C1C=CC=C2.CN1CCOCC1.Cl.CN(C)CCCN=C=NCC>>C(C)(=O)OCCNC(=O)[C@H]1CCCCCC[C@@H](C(N1)=O)CSC(C)=O
[CH3:1][C:2](=[O:3])[O:4][CH2:5][CH2:6][NH2:7].O[C:8](=[O:9])[C@H:10]1[CH2:11][CH2:12][CH2:13][CH2:14][CH2:15][CH2:16][C@H:17]([CH2:18][S:19][C:20]([CH3:21])=[O:22])[C:23](=[O:24])[NH:25]1>>[CH3:1][C:2](=[O:3])[O:4][CH2:5][CH2:6][NH:7][C:8](=[O:9])[C@H:10]1[CH2:11][CH2:12][CH2:13][CH2:14][CH2:15][CH2:16][C@H:17]([CH2:1...
CC(=O)OCCN.CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)O)NC1=O
CC(=O)OCCNC(=O)[C@H]1CCCCCC[C@H](CSC(C)=O)C(=O)N1
null
null
C(Cl)Cl
Acylation
Carboxylic acid with primary amine to amide
37494d655fc476b499cf056f6435518833ae87795aab58744c3c61cc6e2d35e8
1acc31e468ee9ff2d6601bea2d2eb10c464508bb7150073479303b3753dd92b4
O=C1CCCCCCCCN1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[#7:5]-[C:6]=[O;D1;H0:7].[C:8]-[C:9]-[NH2;D1;+0:10]>>[C:4]-[C:3](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[NH;D2;+0:10]-[C:9]-[C:8])-[#7:5]-[C:6]=[O;D1;H0:7]
null
[]
0
CELSIUS
8
HOUR
Trans 3-(acetylthiomethyl)-2-oxo-1-azacyclodecane-10-carboxylic acid (0.15 g, 0.52 mmol), 1-acetoxy-2-aminoethane hydrochloride (0.073 g, 0.52 mmol), 1-hydroxybenzotriazole (0.12 g, 0.52 mmol), and 4-methylmorpholine (0.17 mL, 1.56 mmol) are dissolved in methylene chloride (3.0 mL), and the reaction is cooled to 0° C. ...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary amine
Secondary amide
null
null
C1CCCCNCCCC1
HO-
C(Cl)Cl
0
8
CC(=O)OCCN.CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)O)NC1=O>C(Cl)Cl>CC(=O)OCCNC(=O)[C@H]1CCCCCC[C@H](CSC(C)=O)C(=O)N1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-ee7debe1bbd340b6a45aa36abc48f31c
BrCc1ccccc1.CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)O)NC1=O>>CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)OCc2ccccc2)NC1=O
C(C)(=O)SC[C@@H]1C(N[C@H](CCCCCC1)C(=O)O)=O.C(C1=CC=CC=C1)Br.C([O-])([O-])=O.[Cs+].[Cs+]>>C(C)(=O)SC[C@@H]1C(N[C@H](CCCCCC1)C(=O)OCC1=CC=CC=C1)=O
Br[CH2:17][c:18]1[cH:19][cH:20][cH:21][cH:22][cH:23]1.[CH3:1][C:2](=[O:3])[S:4][CH2:5][C@H:6]1[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][C@H:13]([C:14](=[O:15])[OH:16])[NH:24][C:25]1=[O:26]>>[CH3:1][C:2](=[O:3])[S:4][CH2:5][C@H:6]1[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][C@H:13]([C:14](=[O:15])[O:16][CH2:17][c:...
BrCc1ccccc1.CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)O)NC1=O
CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)OCc2ccccc2)NC1=O
null
null
CN(C=O)C.O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
06c4f868ad4646eea8208ecb83f54ca035dd62d04f0d8101641a4f487f2c695c
8446834f0edd1e71a2dcaffc09b80c7367abf3407263a8998354a2d20c1766bb
O=C1CCCCCCC[C@H](C(=O)OCc2ccccc2)N1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[#7:5]-[C:6]-[C:7](=[O;D1;H0:8])-[OH;D1;+0:9]>>[#7:5]-[C:6]-[C:7](=[O;D1;H0:8])-[O;H0;D2;+0:9]-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
8
HOUR
Trans 3-(acetylthiomethyl)-2-oxo-1-azacyclodecane-10-carboxylic acid (0.15 g, 0.52 mmol) is dissolved in dimethylformamide (2.5 mL). Benzyl bromide (0.062 mL, 0.52 mmol) and cesium carbonate (0.085 g, 0.26 mmol) are added, and the reaction is stirred at room temperature overnight. The reaction is diluted with water, an...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Carboxylic acid
Ester
null
null
C1CCCCNCCCC1.c1ccccc1
HBr
CN(C=O)C.O
null
8
BrCc1ccccc1.CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)O)NC1=O>CN(C=O)C.O>CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)OCc2ccccc2)NC1=O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-dd7e11ffe6e943828cba55b069dff563
CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)N2C(=O)OC[C@H]2Cc2ccccc2)NC1=O.[OH-]>>CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)O)NC1=O
C(C)(=O)SC[C@@H]1C(N[C@H](CCCCCC1)C(=O)N1C(OC[C@H]1CC1=CC=CC=C1)=O)=O.O.[OH-].[Li+]>>C(C)(=O)SC[C@@H]1C(N[C@H](CCCCCC1)C(=O)O)=O
O=C1OC[C@@H](Cc2ccccc2)N1[C:14]([C@H:13]1[CH2:12][CH2:11][CH2:10][CH2:9][CH2:8][CH2:7][C@H:6]([CH2:5][S:4][C:2]([CH3:1])=[O:3])[C:18](=[O:19])[NH:17]1)=[O:15].[OH-:16]>>[CH3:1][C:2](=[O:3])[S:4][CH2:5][C@H:6]1[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][C@H:13]([C:14](=[O:15])[OH:16])[NH:17][C:18]1=[O:19]
CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)N2C(=O)OC[C@H]2Cc2ccccc2)NC1=O.[OH-]
CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)O)NC1=O
null
null
O.O1CCCC1
Acylation
OtherReaction
1600b14cd479cdb7d3a4405c4b04d21fc0e71f247fcc6d65cda537ac98ed7da2
d7ed181e654e8ac131125bbdc5aee5dc90548ccf7549838daacff3be49378f55
O=C1CCCCCCCCN1
O=C1-O-C-[C@@H](-C-c2:c:c:c:c:c:2)-N-1-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[#7:5]-[C:6]=[O;D1;H0:7].[OH-;D0:8]>>[C:4]-[C:3](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[OH;D1;+0:8])-[#7:5]-[C:6]=[O;D1;H0:7]
null
[]
0
CELSIUS
45
MINUTE
The more polar major chiral isomer of N-[[trans 3-(acetylthiomethyl)-2-oxo-1-azacyclodecan-10-yl]-carbonyl]-(R)-4-benzyl-2-oxazolidinone (1.23 g, 2.75 mmol) is dissolved in tetrahydrofuran (45.0 mL) and water (15.0 mL), and the reaction is cooled to 0° C. Lithium hydroxide hydrate (0.116 g, 2.75 mmol) is added, and the...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Substituted dicarboximide
Carboxylic acid
C1COCN1.c1ccccc1
null
C1CCCCNCCCC1
HO-
O.O1CCCC1
0
0.75
CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)N2C(=O)OC[C@H]2Cc2ccccc2)NC1=O.[OH-]>O.O1CCCC1>CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)O)NC1=O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-cd1d5c5dc1cf4e4bb0fa6676330d839a
CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)O)NC1=O.CCOC(=O)[C@@H]1C[C@@H](O)CN1>>CCOC(=O)[C@@H]1C[C@@H](O)CN1C(=O)[C@H]1CCCCCC[C@H](CSC(C)=O)C(=O)N1
C(C)(=O)SC[C@@H]1C(N[C@H](CCCCCC1)C(=O)O)=O.ON1N=NC2=C1C=CC=C2.CN1CCOCC1.Cl.C(C)OC([C@H]1NC[C@@H](C1)O)=O.Cl.CN(C)CCCN=C=NCC>>C(C)OC([C@H]1N(C[C@@H](C1)O)C(=O)[C@H]1CCCCCC[C@@H](C(N1)=O)CSC(C)=O)=O
O[C:12](=[O:13])[C@H:14]1[CH2:15][CH2:16][CH2:17][CH2:18][CH2:19][CH2:20][C@H:21]([CH2:22][S:23][C:24]([CH3:25])=[O:26])[C:27](=[O:28])[NH:29]1.[CH3:1][CH2:2][O:3][C:4](=[O:5])[C@@H:6]1[CH2:7][C@@H:8]([OH:9])[CH2:10][NH:11]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[C@@H:6]1[CH2:7][C@@H:8]([OH:9])[CH2:10][N:11]1[C:12](=[O:13])...
CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)O)NC1=O.CCOC(=O)[C@@H]1C[C@@H](O)CN1
CCOC(=O)[C@@H]1C[C@@H](O)CN1C(=O)[C@H]1CCCCCC[C@H](CSC(C)=O)C(=O)N1
null
null
C(Cl)Cl
Acylation
Acylation of Nitrogen Nucleophiles by Carboxylic Acids
a590d96426a2fbaed42913d9daf8a16471a16de4978200f1d35a30a10009ebe7
c5e4172490b2731ba9322b68af56376edadc31ce0bb9a3dfdea23a1817a852fd
O=C1CCCCCCC[C@H](C(=O)N2CCCC2)N1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[#7:5]-[C:6]=[O;D1;H0:7].[C:8]-[#8:9]-[C:10](=[O;D1;H0:11])-[C:12]1-[C:13]-[C:14]-[C:15]-[NH;D2;+0:16]-1>>[C:4]-[C:3](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[N;H0;D3;+0:16]1-[C:15]-[C:14]-[C:13]-[C:12]-1-[C:10](=[O;D1;H0:11])-[#8:9]-[C:8])-[#7:5]-[C:6]=[O;D1;H0:7]
null
[]
0
CELSIUS
8
HOUR
The enantiomer of trans 3-(acetylthiomethyl)-2-oxo-1-azacyclodecane-10-carboxylic acid of Example 16(0.23 g, 0.80 mmol), 1-hydroxybenzotriazole (0.11 g, 0.80 mmol), 4-methylmorpholine (0.22 mL, 2.0 mmol), and L-hydroxyproline ethyl ester hydrochloride (0.16 g, 0.80 mmol) are dissolved in methylene chloride (5.0 mL), an...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amine
Tertiary amide
C1CCNC1
C1CC[NH]C1
C1CC[NH]C1.C1CCCCNCCCC1
HO-
C(Cl)Cl
0
8
CC(=O)SC[C@H]1CCCCCC[C@H](C(=O)O)NC1=O.CCOC(=O)[C@@H]1C[C@@H](O)CN1>C(Cl)Cl>CCOC(=O)[C@@H]1C[C@@H](O)CN1C(=O)[C@H]1CCCCCC[C@H](CSC(C)=O)C(=O)N1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-b0cbfac023104194ba68e11d16883fb1
CC(C)(C)OC(=O)CC1CCCCCCC(CO)NC1=O.O=C(O)Cc1cccs1>>CC(=O)SCC1CCCCCCC(CC(=O)OC(C)(C)C)C(=O)N1
C(C)(C)(C)OC(=O)CC1C(NC(CCCCCC1)CO)=O.C(C)N(CC)CC.S1C(=CC=C1)CC(=O)O.C(C)N(CC)CC.C1(=CC=C(C=C1)S(=O)(=O)[O-])C.FC1=[N+](C=CC=C1)C>>C(C)(=O)SCC1CCCCCCC(C(N1)=O)CC(=O)OC(C)(C)C
O[CH2:5][CH:6]1[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][CH:13]([CH2:14][C:15](=[O:16])[O:17][C:18]([CH3:19])([CH3:20])[CH3:21])[C:22](=[O:23])[NH:24]1.OC([CH2:1][c:2]1ccc[s:4]1)=[O:3]>>[CH3:1][C:2](=[O:3])[S:4][CH2:5][CH:6]1[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][CH:13]([CH2:14][C:15](=[O:16])[O:17][C:18]([C...
CC(C)(C)OC(=O)CC1CCCCCCC(CO)NC1=O.O=C(O)Cc1cccs1
CC(=O)SCC1CCCCCCC(CC(=O)OC(C)(C)C)C(=O)N1
null
null
C1=CC=CC=C1.CC(=O)C
Protection
OtherReaction
189263d4d19565b9c5c001a81e8abf2a60b1807919ec489920cd4293a1993653
7a83c40990eef465e85ff66652874583517e7c7b69d7750d5f2438fef535f94e
O=C1CCCCCCCCN1
O-C(=[O;H0;D1;+0:1])-[CH2;D2;+0:2]-[c;H0;D3;+0:3]1:[s;H0;D2;+0:4]:c:c:c:1.O-[CH2;D2;+0:5]-[C:6](-[C:7])-[#7:8]-[C:9]=[O;D1;H0:10]>>[C:7]-[C:6](-[CH2;D2;+0:5]-[S;H0;D2;+0:4]-[C;H0;D3;+0:3](-[CH3;D1;+0:2])=[O;H0;D1;+0:1])-[#7:8]-[C:9]=[O;D1;H0:10]
null
[]
null
null
90
MINUTE
3-t-Butoxycarbonylmethyl-10-hydroxymethyl-2-oxo-1-azacyclodecane (0.50 g, 1.67 mmol) is dissolved in acetone (5.0 mL) and benzene (5.0 mL). Triethylamine (0.26 mL, 1.9 mmol) is added, followed by 2-fluoro-1-methylpyridinium toluene-4-sulfonate (0.54 g, 1.9 mmol), and the reaction is stirred at room temperature for 90 m...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary alcohol
Carbo-thioester
c1ccsc1
null
C1CCCCNCCCC1
HO-
C1=CC=CC=C1.CC(=O)C
null
1.5
CC(C)(C)OC(=O)CC1CCCCCCC(CO)NC1=O.O=C(O)Cc1cccs1>C1=CC=CC=C1.CC(=O)C>CC(=O)SCC1CCCCCCC(CC(=O)OC(C)(C)C)C(=O)N1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-9f6126e0435c45d1b9864f1d5abc955e
CCOC(=O)C1CCCCCCC(=O)C(=O)N1.COP(=O)(CC(=O)OC(C)(C)C)OC>>CCOC(=O)C1CCCCCCC(=CC(=O)OC(C)(C)C)C(=O)N1
O=C1NC(CCCCCCC1=O)C(=O)OCC.COP(=O)(OC)CC(=O)OC(C)(C)C>>C(C)(C)(C)OC(=O)C=C1C(NC(CCCCCC1)C(=O)OCC)=O
O=[C:13]1[CH2:12][CH2:11][CH2:10][CH2:9][CH2:8][CH2:7][CH:6]([C:4]([O:3][CH2:2][CH3:1])=[O:5])[NH:24][C:22]1=[O:23].COP(=O)(OC)[CH2:14][C:15](=[O:16])[O:17][C:18]([CH3:19])([CH3:20])[CH3:21]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]1[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][C:13](=[CH:14][C:15](=[O:16])[O:17][C:18]([...
CCOC(=O)C1CCCCCCC(=O)C(=O)N1.COP(=O)(CC(=O)OC(C)(C)C)OC
CCOC(=O)C1CCCCCCC(=CC(=O)OC(C)(C)C)C(=O)N1
null
null
C1(=CC=CC=C1)C.C1CCOC1
C-C Coupling
Wittig with Phosphonium
46e674202571f664c893c061280f1959b89d65a5bd2e0a27e97f4079bf0d5665
79a946b42eb7e7aee42e09efe41630192c1745e07085cd7f7f88cc7b599f9082
[CH]=C1CCCCCCCNC1=O
C-O-P(=O)(-O-C)-[CH2;D2;+0:1]-[C:2](=[O;D1;H0:3])-[#8:4]-[C:5](-[C;D1;H3:6])(-[C;D1;H3:7])-[C;D1;H3:8].O=[C;H0;D3;+0:9](-[C:10]-[C:11])-[C:12](=[O;D1;H0:13])-[#7:14]-[C:15]-[C:16](-[#8:17])=[O;D1;H0:18]>>[#8:17]-[C:16](=[O;D1;H0:18])-[C:15]-[#7:14]-[C:12](=[O;D1;H0:13])-[C;H0;D3;+0:9](=[CH;D2;+0:1]-[C:2](=[O;D1;H0:3])-...
null
[]
null
null
25
MINUTE
Potassium hexamethyldisilylamide (40.5 mL of a 0.58M solution in toluene, 23.5 mmol) is added to THF (60 mL), and then cooled to 0° C. t-Butyl dimethylphosphonoacetate (4.6 mL, 23.5 mmol) is added dropwise, and the reaction is warmed to room temperature and stirred for 25 minutes. Ethyl 2,3-di-oxo-1-azacyclodecane-10-c...
10.6084/m9.figshare.5104873.v1
null
Ketone.Ester
Ester
C1CCCCNCCCC1
C1CCCCNCCCC1
C1CCCCNCCCC1
HO-
C1(=CC=CC=C1)C.C1CCOC1
null
0.416667
CCOC(=O)C1CCCCCCC(=O)C(=O)N1.COP(=O)(CC(=O)OC(C)(C)C)OC>C1(=CC=CC=C1)C.C1CCOC1>CCOC(=O)C1CCCCCCC(=CC(=O)OC(C)(C)C)C(=O)N1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-17a0cf59456c4baa92e9560f5124e23f
CCOC(=O)C1CCCCCCC(=CC(=O)OC(C)(C)C)C(=O)N1>>CCOC(=O)C1CCCCCCC(CC(=O)OC(C)(C)C)C(=O)N1
C(C)(C)(C)OC(=O)C=C1C(NC(CCCCCC1)C(=O)OCC)=O>>C(C)(C)(C)OC(=O)CC1C(NC(CCCCCC1)C(=O)OCC)=O
[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]1[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][C:13](=[CH:14][C:15](=[O:16])[O:17][C:18]([CH3:19])([CH3:20])[CH3:21])[C:22](=[O:23])[NH:24]1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]1[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][CH:13]([CH2:14][C:15](=[O:16])[O:17][C:18]([CH3:19])([C...
CCOC(=O)C1CCCCCCC(=CC(=O)OC(C)(C)C)C(=O)N1
CCOC(=O)C1CCCCCCC(CC(=O)OC(C)(C)C)C(=O)N1
null
[Pd]
C(C)(=O)OCC
Reduction
Hydrogenation (double to single)
c528462945509c32a83b30347f7f4ef4d89ae59c56cc702e111e9c5086d00dff
9a50abf8d2e4cd9195d7a0cadbe97483a261a81cf70b653cfddd5ecf76d383a6
O=C1CCCCCCCCN1
[#8:1]-[C:2](=[O;D1;H0:3])-[C:4]-[#7:5]-[C:6](=[O;D1;H0:7])-[C;H0;D3;+0:8](=[CH;D2;+0:9]-[C:10](=[O;D1;H0:11])-[#8:12]-[C:13](-[C;D1;H3:14])(-[C;D1;H3:15])-[C;D1;H3:16])-[C:17]-[C:18]>>[#8:1]-[C:2](=[O;D1;H0:3])-[C:4]-[#7:5]-[C:6](=[O;D1;H0:7])-[CH;D3;+0:8](-[CH2;D2;+0:9]-[C:10](=[O;D1;H0:11])-[#8:12]-[C:13](-[C;D1;H3:...
null
[]
null
null
4.5
HOUR
Ethyl 3-t-butoxycarbonylmethylidene-2-oxo-1-azacyclodecane-10-carboxylate (2.85 g, 8.4 mmol) is dissolved in ethyl acetate (75 mL). 10% Pd/C (2.0 g) is added, and the reaction is stirred under an atmosphere of hydrogen for 4.5 hours. The reaction is filtered through Celite, and the solvent is removed. The crude product...
10.6084/m9.figshare.5104873.v1
null
Ester
Ester
C1CCCCNCCCC1
C1CCCCNCCCC1
C1CCCCNCCCC1
null
[Pd].C(C)(=O)OCC
null
4.5
CCOC(=O)C1CCCCCCC(=CC(=O)OC(C)(C)C)C(=O)N1>[Pd].C(C)(=O)OCC>CCOC(=O)C1CCCCCCC(CC(=O)OC(C)(C)C)C(=O)N1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-429516784f194c80be8e088df5ef86d4
CCOC(=O)C1CCCCCCC(CC(=O)OC(C)(C)C)C(=O)N1>>CC(C)(C)OC(=O)CC1CCCCCCC(CO)NC1=O
C(C)(C)(C)OC(=O)CC1C(NC(CCCCCC1)C(=O)OCC)=O.[BH4-].[Na+].CO>>C(C)(C)(C)OC(=O)CC1C(NC(CCCCCC1)CO)=O
CCO[C:17]([CH:16]1[CH2:15][CH2:14][CH2:13][CH2:12][CH2:11][CH2:10][CH:9]([CH2:8][C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[C:20](=[O:21])[NH:19]1)=[O:18]>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[CH2:8][CH:9]1[CH2:10][CH2:11][CH2:12][CH2:13][CH2:14][CH2:15][CH:16]([CH2:17][OH:18])[NH:19][C:20]1=[O:21]
CCOC(=O)C1CCCCCCC(CC(=O)OC(C)(C)C)C(=O)N1
CC(C)(C)OC(=O)CC1CCCCCCC(CO)NC1=O
null
null
C(C)(C)(C)O
Reduction
Reduction of ester to primary alcohol
21d61543c6ec8a8cebe1b3ef55ef3dd20acbf79a4f1c12a7fb51e32be7a3248a
1fbcd628a0426673c5d10aa49a977cd2d1ae02a8cdf57bbb10d94aa03a94e937
O=C1CCCCCCCCN1
C-C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[C:3](-[C:4])-[#7:5]-[C:6]=[O;D1;H0:7]>>[C:4]-[C:3](-[CH2;D2;+0:1]-[OH;D1;+0:2])-[#7:5]-[C:6]=[O;D1;H0:7]
null
[]
55
CELSIUS
1
HOUR
The major isomer of ethyl 3-t-butoxycarbonylmethyl-2-oxo-1-azacyclodecane-10-carboxylate (0.68 g, 2.0 mmol) is dissolved in t-butanol (10 mL). Sodium borohydride (0.23 g, 6.0 mmol) is added and the reaction is warmed to 55° C. Methanol (2.0 mL) is added over a twenty minute period, and the reaction is kept at 55° C. fo...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary alcohol
null
null
C1CCCCNCCCC1
HO-
C(C)(C)(C)O
55
1
CCOC(=O)C1CCCCCCC(CC(=O)OC(C)(C)C)C(=O)N1>C(C)(C)(C)O>CC(C)(C)OC(=O)CC1CCCCCCC(CO)NC1=O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-3ff5ad5cf75d47f1b22289091515d997
CC(C)(C)OC(=O)CC1CCCCCCC(CS)NC1=O>>O=C(O)CC1CCCCCCC(CS)NC1=O
SCC1CCCCCCC(C(N1)=O)CC(=O)OC(C)(C)C>>SCC1CCCCCCC(C(N1)=O)CC(=O)O
CC(C)(C)[O:3][C:2](=[O:1])[CH2:4][CH:5]1[CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH:12]([CH2:13][SH:14])[NH:15][C:16]1=[O:17]>>[O:1]=[C:2]([OH:3])[CH2:4][CH:5]1[CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH:12]([CH2:13][SH:14])[NH:15][C:16]1=[O:17]
CC(C)(C)OC(=O)CC1CCCCCCC(CS)NC1=O
O=C(O)CC1CCCCCCC(CS)NC1=O
null
null
C(Cl)Cl
Deprotection
Deprotection of carboxylic acid
152e5537e48c95b4a3e767536b0f9f68d1308e5f484070828ab5ed951805157a
7f019d4cfe9b3036d0a2d3a3209aa0e1fcb05418ebee15a4be5e125d315d5f01
O=C1CCCCCCCCN1
C-C(-C)(-C)-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
null
[]
null
null
8
HOUR
10-Mercaptomethyl-3-t-butoxycarbonylmethyl-2-oxo-1-azacyclodecane (0.21 g, 0.69 mmol) is dissolved in methylene chloride (15 mL). Gaseous hydrogen chloride is bubbled through the solvent for 15 minutes, and then the reaction is sealed and stirred overnight. The solvent is evaporated the next day to give 10-mercaptometh...
10.6084/m9.figshare.5104873.v1
null
Ester.Boc
Carboxylic acid
null
null
C1CCCCNCCCC1
Other
C(Cl)Cl
null
8
CC(C)(C)OC(=O)CC1CCCCCCC(CS)NC1=O>C(Cl)Cl>O=C(O)CC1CCCCCCC(CS)NC1=O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-4ea35438c1a34afdb409c8baaa96ef06
CCOC(=O)CC(CCCCCCCCCCC(CC(=O)OCC)C(=O)OCc1ccccc1)NC(=O)OC(C)(C)C>>CCOC(=O)CC(CCCCCCCCCCC(CC(=O)OCC)C(=O)O)NC(=O)OC(C)(C)C
C(C)(C)(C)OC(=O)NC(CC(=O)OCC)CCCCCCCCCCC(CC(=O)OCC)C(=O)OCC1=CC=CC=C1>>C(C)(C)(C)OC(=O)NC(CC(=O)OCC)CCCCCCCCCCC(CC(=O)OCC)C(=O)O
c1ccc(C[O:27][C:25]([CH:18]([CH2:17][CH2:16][CH2:15][CH2:14][CH2:13][CH2:12][CH2:11][CH2:10][CH2:9][CH2:8][CH:7]([CH2:6][C:4]([O:3][CH2:2][CH3:1])=[O:5])[NH:28][C:29](=[O:30])[O:31][C:32]([CH3:33])([CH3:34])[CH3:35])[CH2:19][C:20](=[O:21])[O:22][CH2:23][CH3:24])=[O:26])cc1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][CH:7]...
CCOC(=O)CC(CCCCCCCCCCC(CC(=O)OCC)C(=O)OCc1ccccc1)NC(=O)OC(C)(C)C
CCOC(=O)CC(CCCCCCCCCCC(CC(=O)OCC)C(=O)O)NC(=O)OC(C)(C)C
null
[Pd]
C(C)(=O)OCC
Deprotection
Ester saponification (alkyl deprotection)
86a971d3e4f88009ab4c98512e9f1deb51b2f0ce5cbd068cc61ae878c1e58e2a
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
null
[C:1]-[C:2](=[O;D1;H0:3])-[O;H0;D2;+0:4]-C-c1:c:c:c:c:c:1>>[C:1]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:4]
null
[]
null
null
2
HOUR
Diethyl 2-t-butoxycarbonylamino-13-benzyloxycarbonyl-1,14-tetradecanedicarboxylate (5.0 g, 8.87 mmol) is dissolved in ethyl acetate (150.0 mL), and 10% Pd-C (2.6 g) is added. The reaction flask is put under an atmosphere of hydrogen and stirred for 2 hours. The product is then filtered through a pad of Celite, and the ...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
c1ccccc1
null
null
Other
[Pd].C(C)(=O)OCC
null
2
CCOC(=O)CC(CCCCCCCCCCC(CC(=O)OCC)C(=O)OCc1ccccc1)NC(=O)OC(C)(C)C>[Pd].C(C)(=O)OCC>CCOC(=O)CC(CCCCCCCCCCC(CC(=O)OCC)C(=O)O)NC(=O)OC(C)(C)C
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-856e1c74c5fa4bfaa718c434d3d2dcd8
CCOC(=O)CC(CCCCCCCCCCC(CC(=O)OCC)C(=O)O)NC(=O)OC(C)(C)C.ClCCl>>CCOC(=O)CC(N)CCCCCCCCCCC(CC(=O)OCC)C(=O)O.Cl
C(C)(C)(C)OC(=O)NC(CC(=O)OCC)CCCCCCCCCCC(CC(=O)OCC)C(=O)O.C(Cl)Cl>>Cl.NC(CC(=O)OCC)CCCCCCCCCCC(CC(=O)OCC)C(=O)O
CC(C)(C)OC(=O)[NH:8][CH:7]([CH2:6][C:4]([O:3][CH2:2][CH3:1])=[O:5])[CH2:9][CH2:10][CH2:11][CH2:12][CH2:13][CH2:14][CH2:15][CH2:16][CH2:17][CH2:18][CH:19]([CH2:20][C:21](=[O:22])[O:23][CH2:24][CH3:25])[C:26](=[O:27])[OH:28].ClC[Cl:29]>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][CH:7]([NH2:8])[CH2:9][CH2:10][CH2:11][CH2:12]...
CCOC(=O)CC(CCCCCCCCCCC(CC(=O)OCC)C(=O)O)NC(=O)OC(C)(C)C.ClCCl
CCOC(=O)CC(N)CCCCCCCCCCC(CC(=O)OCC)C(=O)O.Cl
null
null
null
Miscellaneous
OtherReaction
20ca630092c9d0b186049ded8d4724cd41b8cec5a9770e37b4b0e3b10fb39ea3
b777363b1194e165a6e8ffea7fe0d21d29ef4e8f6652e2bc49cad8e827d3c935
null
C-C(-C)(-C)-O-C(=O)-[NH;D2;+0:1]-[C:2](-[C:3])-[C:4]-[C:5](-[#8:6])=[O;D1;H0:7].Cl-C-[Cl;H0;D1;+0:8]>>[#8:6]-[C:5](=[O;D1;H0:7])-[C:4]-[C:2](-[C:3])-[NH2;D1;+0:1].[ClH;D0;+0:8]
null
[]
null
null
2.5
HOUR
Diethyl 2-t-butoxycarbonylamino-13-carboxy-1,14-tetradecanedicarboxylate (3.98 g, 8.40 mmol) is dissolved in methylene chloride (150.0 mL), and hydrogen chloride gas is bubbled through the solution for 15 minutes. The sealed reaction is stirred for 2.5 hours, and then the solvent is evaporated to give diethyl 2-amino-1...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary halide.Carbamic ester.Ether.Boc
Primary amine
null
null
null
HCl
null
null
2.5
CCOC(=O)CC(CCCCCCCCCCC(CC(=O)OCC)C(=O)O)NC(=O)OC(C)(C)C.ClCCl>>CCOC(=O)CC(N)CCCCCCCCCCC(CC(=O)OCC)C(=O)O.Cl
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-951c6a1597cb49a28e3182feddd4d406
CCOC(=O)C1CCCCCCCCCCC(C(=O)OCC)C(=O)N1>>O=C(O)C1CCCCCCCCCCC(C(=O)O)C(=O)N1
Cl.O=C1NC(CCCCCCCCCCC1C(=O)OCC)C(=O)OCC.[OH-].[Na+]>>O=C1NC(CCCCCCCCCCC1C(=O)O)C(=O)O
CC[O:3][C:2](=[O:1])[CH:4]1[CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][CH2:13][CH2:14][CH:15]([C:16](=[O:17])[O:18]CC)[C:19](=[O:20])[NH:21]1>>[O:1]=[C:2]([OH:3])[CH:4]1[CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][CH2:13][CH2:14][CH:15]([C:16](=[O:17])[OH:18])[C:19](=[O:20])[NH:21]1
CCOC(=O)C1CCCCCCCCCCC(C(=O)OCC)C(=O)N1
O=C(O)C1CCCCCCCCCCC(C(=O)O)C(=O)N1
null
null
C(C)O
Deprotection
OtherReaction
6e62db7aac546f574bcfb83067ba8906c30fcbfedfc37aa16b5eaad33833f45a
ed5fed81ba501ef41c88831ec6b9463b899bfdd0815c4145ae51c79addb226d0
O=C1CCCCCCCCCCCCN1
C-C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[C:4]-[C:5](=[O;D1;H0:6])-[#7:7]-[C:8]-[C:9](=[O;D1;H0:10])-[O;H0;D2;+0:11]-C-C>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[C:4]-[C:5](=[O;D1;H0:6])-[#7:7]-[C:8]-[C:9](=[O;D1;H0:10])-[OH;D1;+0:11]
null
[]
null
null
3
HOUR
Diethyl 2-oxo-1-azacyclotetradecane-3,14-dicarboxylate (1.14 g, 3.2 mmol; mixture of both diastereomers) is dissolved in ethanol (32.0 mL). Sodium hydroxide (9.6 mL of a 1N aqueous solution, 9.6 mmol) is added dropwise, and the solution is stirred at room temperature for 3 hours. The reaction is then acidified to pH 3 ...
10.6084/m9.figshare.5104873.v1
null
Ester.Ester
Carboxylic acid.Carboxylic acid
null
null
C1CCCCCCNCCCCCC1
Other
C(C)O
null
3
CCOC(=O)C1CCCCCCCCCCC(C(=O)OCC)C(=O)N1>C(C)O>O=C(O)C1CCCCCCCCCCC(C(=O)O)C(=O)N1
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-d4e78d67f9574f95b9763ece1f167e82
O=C(O)C1CCCCCCCCCCC(C(=O)O)C(=O)N1>>C=C1CCCCCCCCCCC(C(=O)O)NC1=O
Cl.N1CCCCC1.O=C1NC(CCCCCCCCCCC1C(=O)O)C(=O)O.C=O>>C=C1C(NC(CCCCCCCCCC1)C(=O)O)=O
O=[C:1](O)[CH:2]1[CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][CH:13]([C:14](=[O:15])[OH:16])[C:18](=[O:19])[NH:17]1>>[CH2:1]=[C:2]1[CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][CH:13]([C:14](=[O:15])[OH:16])[NH:17][C:18]1=[O:19]
O=C(O)C1CCCCCCCCCCC(C(=O)O)C(=O)N1
C=C1CCCCCCCCCCC(C(=O)O)NC1=O
null
null
N1=CC=CC=C1
Miscellaneous
OtherReaction
606ce5b982dd54d5ddad914cad200a87e4e95b65ba2c1a08c497beef81ebff6f
52fef7a0b69b8402c1bf3297cc4d8b52084cb5f5aab54ba262b4908f5ccbe01d
C=C1CCCCCCCCCCCNC1=O
O-[C;H0;D3;+0:1](=O)-[CH;D3;+0:2](-[C:3]-[C:4])-[NH;D2;+0:5]-[C;H0;D3;+0:6](=[O;D1;H0:7])-[CH;D3;+0:8](-[C:9](=[O;D1;H0:10])-[O;D1;H1:11])-[C:12]-[C:13]>>[C:13]-[C:12]-[CH;D3;+0:8](-[C:9](=[O;D1;H0:10])-[O;D1;H1:11])-[NH;D2;+0:5]-[C;H0;D3;+0:6](=[O;D1;H0:7])-[C;H0;D3;+0:2](=[CH2;D1;+0:1])-[C:3]-[C:4]
null
[]
65
CELSIUS
null
null
2-oxo-1-azacyclotetradecane-3,14-dicarboxylic acid (0.868 g, 2.9 mmol) is dissolved in pyridine (15.0 mL). Piperidine (0.060 mL, 0.59 mmol) is added, followed by paraformaldehyde (0.133 g, 4.43 mmol), and the reaction is heated to 65° C. for 4 hours. The reaction is then cooled to 0° C., and concentrated hydrochloric a...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Secondary amide
Secondary amide.Vinyl
C1CCCCCCNCCCCCC1
C1CCCCCCNCCCCCC1
C1CCCCCCNCCCCCC1
Other
N1=CC=CC=C1
65
null
O=C(O)C1CCCCCCCCCCC(C(=O)O)C(=O)N1>N1=CC=CC=C1>C=C1CCCCCCCCCCC(C(=O)O)NC1=O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-f8fa4f864ba6411e93d231ab3c63d6ce
BrCCCCCCCBr.COC(=O)CC(=O)OC(C)(C)C>>COC(=O)C(CCCCCCCBr)C(=O)OC(C)(C)C
BrCCCCCCCBr.[H-].[Na+].C(CC(=O)OC)(=O)OC(C)(C)C>>BrCCCCCCCC(C(=O)OC(C)(C)C)C(=O)OC
Br[CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][Br:13].[CH3:1][O:2][C:3](=[O:4])[CH2:5][C:14](=[O:15])[O:16][C:17]([CH3:18])([CH3:19])[CH3:20]>>[CH3:1][O:2][C:3](=[O:4])[CH:5]([CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][Br:13])[C:14](=[O:15])[O:16][C:17]([CH3:18])([CH3:19])[CH3:20]
BrCCCCCCCBr.COC(=O)CC(=O)OC(C)(C)C
COC(=O)C(CCCCCCCBr)C(=O)OC(C)(C)C
null
null
CN(C=O)C
C-C Coupling
OtherReaction
8175b6573d6439ec7ccc45bf6b48843ab56b46dccfc6504384c4766d09f35cc7
d1817e44576d3a158547867a56245217a593d4f828a6d6dfaa8ed11276894e44
null
Br-[CH2;D2;+0:1]-[C:2]-[C:3].[C;D1;H3:4]-[C:5](-[C;D1;H3:6])(-[C;D1;H3:7])-[#8:8]-[C:9](=[O;D1;H0:10])-[CH2;D2;+0:11]-[C:12](=[O;D1;H0:13])-[#8:14]-[C;D1;H3:15]>>[C:3]-[C:2]-[CH2;D2;+0:1]-[CH;D3;+0:11](-[C:9](=[O;D1;H0:10])-[#8:8]-[C:5](-[C;D1;H3:4])(-[C;D1;H3:6])-[C;D1;H3:7])-[C:12](=[O;D1;H0:13])-[#8:14]-[C;D1;H3:15]
null
[]
null
null
3
HOUR
Sodium hydride (3.04 g of a 50% oil dispersion, 127 mmol) is suspended in dimethylformamide (300 ml) and the suspension is cooled to 0° C. t-Butyl methyl malonate (20.08 g, 115 mmol) is added dropwise slowly and the reaction mixture is warmed to room temperature. 1,7-Dibromoheptane (29.75 g, 115 mmol) is added dropwise...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Ester.Ester
Ester.Ester
null
null
null
HBr
CN(C=O)C
null
3
BrCCCCCCCBr.COC(=O)CC(=O)OC(C)(C)C>CN(C=O)C>COC(=O)C(CCCCCCCBr)C(=O)OC(C)(C)C
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-2f96668fb4f34f4cb203add2e1dbf0d7
COC(=O)C(CCCCCCCBr)C(=O)OC(C)(C)C.[I-]>>COC(=O)C(CCCCCCCI)C(=O)OC(C)(C)C
BrCCCCCCCC(C(=O)OC(C)(C)C)C(=O)OC.[I-].[Na+]>>ICCCCCCCC(C(=O)OC(C)(C)C)C(=O)OC
Br[CH2:12][CH2:11][CH2:10][CH2:9][CH2:8][CH2:7][CH2:6][CH:5]([C:3]([O:2][CH3:1])=[O:4])[C:14](=[O:15])[O:16][C:17]([CH3:18])([CH3:19])[CH3:20].[I-:13]>>[CH3:1][O:2][C:3](=[O:4])[CH:5]([CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][I:13])[C:14](=[O:15])[O:16][C:17]([CH3:18])([CH3:19])[CH3:20]
COC(=O)C(CCCCCCCBr)C(=O)OC(C)(C)C.[I-]
COC(=O)C(CCCCCCCI)C(=O)OC(C)(C)C
null
null
CC(=O)C
Functional Group Interconversion
OtherReaction
e944a2acb95a43a23818321f2ac2f96ba2f2b8d34f52c1cfd1e3802d2403177f
e2ca6f9fe1078a3836d617896a4e5cc310fb155ca459b021e2b549b3e61f1df7
null
Br-[CH2;D2;+0:1]-[C:2]-[C:3].[I-;H0;D0:4]>>[C:3]-[C:2]-[CH2;D2;+0:1]-[I;H0;D1;+0:4]
null
[]
null
null
null
null
t-Butyl methyl 7-bromoheptylmalonate (8.81 g, 25.1 mmol) is dissolved in acetone (50 ml). Sodium iodide (3.7 g, 25.1 mmol) is added and the mixture is stirred at reflux for 2 hours. The reaction mixture is filtered and the filtrate is concentrated to dryness. The residue is dissolved in methylene chloride and filtered ...
10.6084/m9.figshare.5104873.v1
null
Primary halide
Primary halide
null
null
null
Br-
CC(=O)C
null
null
COC(=O)C(CCCCCCCBr)C(=O)OC(C)(C)C.[I-]>CC(=O)C>COC(=O)C(CCCCCCCI)C(=O)OC(C)(C)C
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-13270cd53a13413d86e4aa414a30ff1f
COC(=O)CC(CCCCCCCSC[C@H](N)CC(=O)OC)C(=O)OC(C)(C)C.ClCCl>>COC(=O)CC(CCCCCCCSC[C@H](N)CC(=O)OC)C(=O)O.Cl
N[C@H](CC(=O)OC)CSCCCCCCCC(CC(=O)OC)C(=O)OC(C)(C)C.C(Cl)Cl>>Cl.N[C@H](CC(=O)OC)CSCCCCCCCC(CC(=O)OC)C(=O)O
CC(C)(C)[O:25][C:23]([CH:6]([CH2:5][C:3]([O:2][CH3:1])=[O:4])[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][CH2:13][S:14][CH2:15][C@H:16]([NH2:17])[CH2:18][C:19](=[O:20])[O:21][CH3:22])=[O:24].ClC[Cl:26]>>[CH3:1][O:2][C:3](=[O:4])[CH2:5][CH:6]([CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][CH2:13][S:14][CH2:15][C@H:16]([...
COC(=O)CC(CCCCCCCSC[C@H](N)CC(=O)OC)C(=O)OC(C)(C)C.ClCCl
COC(=O)CC(CCCCCCCSC[C@H](N)CC(=O)OC)C(=O)O.Cl
null
null
null
Miscellaneous
OtherReaction
1bdde8ea72e11cfbcc043bc42d0b84bb99dcaa21c1178d188748f396a79f95e1
24c87f8d54dd79ab3c2ede7dc82b7333299b3ef9471862dc0277670fba8260f4
null
C-C(-C)(-C)-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4].Cl-C-[Cl;H0;D1;+0:5]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1].[ClH;D0;+0:5]
null
[]
null
null
2
HOUR
Dimethyl (2R)-2-amino-12-t-butoxycarbonyl-4-thia-1,13-tridecanedicarboxylate (3.39 g, 8.36 mmol) is dissolved in methylene chloride (50 ml) and hydrogen chloride gas is bubbled through the solution for 5 minutes. The reaction mixture is stirred for 2 hours at room temperature. The solvent is evaporated to give dimethyl...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary halide.Ester.Boc
Carboxylic acid
null
null
null
HCl
null
null
2
COC(=O)CC(CCCCCCCSC[C@H](N)CC(=O)OC)C(=O)OC(C)(C)C.ClCCl>>COC(=O)CC(CCCCCCCSC[C@H](N)CC(=O)OC)C(=O)O.Cl
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-d95927d178064a35970f180e99ed80b8
COC(=O)C1CCCCCCCSC[C@@H](C(=O)OC)NC1=O>>O=C(O)C1CCCCCCCSC[C@@H](C(=O)O)NC1=O
COC(=O)C1C(N[C@@H](CSCCCCCCC1)C(=O)OC)=O.[OH-].[Na+]>>C(=O)(O)C1C(N[C@@H](CSCCCCCCC1)C(=O)O)=O
C[O:3][C:2](=[O:1])[CH:4]1[CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][S:12][CH2:13][C@@H:14]([C:15](=[O:16])[O:17]C)[NH:18][C:19]1=[O:20]>>[O:1]=[C:2]([OH:3])[CH:4]1[CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][S:12][CH2:13][C@@H:14]([C:15](=[O:16])[OH:17])[NH:18][C:19]1=[O:20]
COC(=O)C1CCCCCCCSC[C@@H](C(=O)OC)NC1=O
O=C(O)C1CCCCCCCSC[C@@H](C(=O)O)NC1=O
null
null
CO
Deprotection
OtherReaction
6e62db7aac546f574bcfb83067ba8906c30fcbfedfc37aa16b5eaad33833f45a
ed5fed81ba501ef41c88831ec6b9463b899bfdd0815c4145ae51c79addb226d0
O=C1CCCCCCCCSCCN1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[C:4]-[#7:5]-[C:6](=[O;D1;H0:7])-[C:8]-[C:9](=[O;D1;H0:10])-[O;H0;D2;+0:11]-C>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[C:4]-[#7:5]-[C:6](=[O;D1;H0:7])-[C:8]-[C:9](=[O;D1;H0:10])-[OH;D1;+0:11]
null
[]
null
null
4
HOUR
Methyl (3R)-6-methoxycarbonyl-5oxo-1-thia-4-azacyclotridecane-3-carboxylate (2.39 g, 7.21 mmol) is suspended in methanol (75 ml) and 1N sodium hydroxide (22.0 ml, 22.0 mmol) is added. The mixture is stirred for 4 hours at room temperature. The solvent is evaporated and the residue is dissolved in water (150 ml). The aq...
10.6084/m9.figshare.5104873.v1
null
Ester.Ester
Carboxylic acid.Carboxylic acid
null
null
C1CCCCNCCSCCCC1
Other
CO
null
4
COC(=O)C1CCCCCCCSC[C@@H](C(=O)OC)NC1=O>CO>O=C(O)C1CCCCCCCSC[C@@H](C(=O)O)NC1=O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-65e3bf11fde04d758153eba4550a656c
O=C(O)C1CCCCCCCSC[C@@H](C(=O)O)NC1=O>>C=C1CCCCCCCSC[C@@H](C(=O)O)NC1=O
Cl.N1CCCCC1.C(=O)(O)C1C(N[C@@H](CSCCCCCCC1)C(=O)O)=O.C=O>>C=C1C(N[C@@H](CSCCCCCCC1)C(=O)O)=O
O=[C:1](O)[CH:2]1[CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][S:10][CH2:11][C@@H:12]([C:13](=[O:14])[OH:15])[NH:16][C:17]1=[O:18]>>[CH2:1]=[C:2]1[CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][S:10][CH2:11][C@@H:12]([C:13](=[O:14])[OH:15])[NH:16][C:17]1=[O:18]
O=C(O)C1CCCCCCCSC[C@@H](C(=O)O)NC1=O
C=C1CCCCCCCSC[C@@H](C(=O)O)NC1=O
null
null
N1=CC=CC=C1
Miscellaneous
OtherReaction
ff8c773c54c3749caf140ff97e4a140e15d8bb81dd68b71552c083576e448385
f72397e2bf1ed63b336420ad8491805dec3139bd28093f1f8ae2a191ad5039cf
C=C1CCCCCCCSCCNC1=O
O-[C;H0;D3;+0:1](=O)-[CH;D3;+0:2](-[C:3]-[C:4])-[C:5](=[O;D1;H0:6])-[#7:7]-[C:8]-[C:9](=[O;D1;H0:10])-[O;D1;H1:11]>>[C:4]-[C:3]-[C;H0;D3;+0:2](=[CH2;D1;+0:1])-[C:5](=[O;D1;H0:6])-[#7:7]-[C:8]-[C:9](=[O;D1;H0:10])-[O;D1;H1:11]
null
[]
65
CELSIUS
2
HOUR
(3R)-6-Carboxy-5-oxo-1-thia-4-azacyclotridecane -3-carboxylic acid (1.71 g, 5.64 mmol) is dissolved in pyridine (20 ml) and piperidine (0.096 g, 1.13 mmol) is added followed by paraformaldehyde (0.25 g, 8.46 mmol). The mixture is heated to 65° C. and stirred for 2 hours. The mixture is cooled to room temperature, poure...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Vinyl
C1CCCCNCCSCCCC1
C1CCCCNCCSCCCC1
C1CCCCNCCSCCCC1
Other
N1=CC=CC=C1
65
2
O=C(O)C1CCCCCCCSC[C@@H](C(=O)O)NC1=O>N1=CC=CC=C1>C=C1CCCCCCCSC[C@@H](C(=O)O)NC1=O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-8a5922e693b148e3b13ed802c0393b83
COC(=O)[C@@H]1CSCCCCCCCC(CSC(C)=O)C(=O)N1>>O=C1N[C@H](C(=O)O)CSCCCCCCCC1CS
C(C)(=O)SCC1C(N[C@@H](CSCCCCCCC1)C(=O)OC)=O.O.[OH-].[Li+].Cl>>SCC1C(N[C@@H](CSCCCCCCC1)C(=O)O)=O
CC(=O)[S:19][CH2:18][CH:17]1[C:2](=[O:1])[NH:3][C@H:4]([C:5](=[O:6])[O:7]C)[CH2:8][S:9][CH2:10][CH2:11][CH2:12][CH2:13][CH2:14][CH2:15][CH2:16]1>>[O:1]=[C:2]1[NH:3][C@H:4]([C:5](=[O:6])[OH:7])[CH2:8][S:9][CH2:10][CH2:11][CH2:12][CH2:13][CH2:14][CH2:15][CH2:16][CH:17]1[CH2:18][SH:19]
COC(=O)[C@@H]1CSCCCCCCCC(CSC(C)=O)C(=O)N1
O=C1N[C@H](C(=O)O)CSCCCCCCCC1CS
null
null
null
Reduction
OtherReaction
1bcd8cbb2f136b4bcba1690e9ba45c4e43c89ba76f0e22de82a7d3fe318c82a9
5654c46fe4cb226f88ec3c899c7f9be1825c357673ea686958f9ef4883ee1db3
O=C1CCCCCCCCSCCN1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[C:4]-[#7:5]-[C:6](=[O;D1;H0:7])-[C:8]-[C:9]-[S;H0;D2;+0:10]-C(-C)=O>>[O;D1;H0:7]=[C:6](-[#7:5]-[C:4]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:1])-[C:8]-[C:9]-[SH;D1;+0:10]
null
[]
null
null
3
HOUR
Methyl (3R)-6-(acetylthiomethyl)-5-oxo-1-thia-4-azacyclotridecane-3-carboxylate (Isomer B) (0.16 g, 0.44 mmol) is partially dissolved in nitrogen degassed tetrahydrofuran (10 ml) and water (5 ml). Lithium hydroxide monohydrate (0.056 g, 1.33 mmol) is added and the mixture is stirred at room temperature for 3 hours. The...
10.6084/m9.figshare.5104873.v1
null
Ester.Carbo-thioester
Carboxylic acid.Aliphatic thiol
null
null
C1CCCCNCCSCCCC1
HO-
null
null
3
COC(=O)[C@@H]1CSCCCCCCCC(CSC(C)=O)C(=O)N1>>O=C1N[C@H](C(=O)O)CSCCCCCCCC1CS
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-2e9b771a72464fd2a4cf50637c02194b
C=C1CCCCCCCSC[C@@H](C(=O)O)NC1=O.CCO>>C=C1CCCCCCCSC[C@@H](C(=O)OCC)NC1=O
C=C1C(N[C@@H](CSCCCCCCC1)C(=O)O)=O.C(C)O>>C=C1C(N[C@@H](CSCCCCCCC1)C(=O)OCC)=O
[CH2:1]=[C:2]1[CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][S:10][CH2:11][C@@H:12]([C:13](=[O:14])[OH:15])[NH:18][C:19]1=[O:20].O[CH2:16][CH3:17]>>[CH2:1]=[C:2]1[CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][S:10][CH2:11][C@@H:12]([C:13](=[O:14])[O:15][CH2:16][CH3:17])[NH:18][C:19]1=[O:20]
C=C1CCCCCCCSC[C@@H](C(=O)O)NC1=O.CCO
C=C1CCCCCCCSC[C@@H](C(=O)OCC)NC1=O
null
null
null
Heteroatom Alkylation and Arylation
Esterification of Carboxylic Acids
3f9a9ace480b666da05fcfe5450d12b5c1ea5b0d435c195e1dd4bd20281604bb
dcbf04ec563ed0e9dfc79070490a028958024079a671c385858bb18cc8ec995a
C=C1CCCCCCCSCCNC1=O
O-[CH2;D2;+0:1]-[C;D1;H3:2].[#7:3]-[C:4]-[C:5](=[O;D1;H0:6])-[OH;D1;+0:7]>>[#7:3]-[C:4]-[C:5](=[O;D1;H0:6])-[O;H0;D2;+0:7]-[CH2;D2;+0:1]-[C;D1;H3:2]
null
[]
null
null
8
HOUR
(3R)-6-Methylidene-5-oxo-1-thia-4-azacyclotridecane-3-carboxylic acid (0.16 g), 0.62 mmol) is dissolved in ethanol (5 ml) and hydrogen chloride gas is bubbled through the solution for 5 minutes. The solution is stirred overnight at room temperature and the solvent is evaporated to give ethyl (3R)-6-methylidene-5-oxo-1-...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Primary alcohol
Ester
null
null
C1CCCCNCCSCCCC1
HO-
null
null
8
C=C1CCCCCCCSC[C@@H](C(=O)O)NC1=O.CCO>>C=C1CCCCCCCSC[C@@H](C(=O)OCC)NC1=O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-2c4718ae54194d608dd1f148f41104d9
BrCc1ccccc1.CC(=O)SCC1CCCCCCCSC[C@@H](C(=O)O)NC1=O>>CC(=O)SCC1CCCCCCCSC[C@@H](C(=O)OCc2ccccc2)NC1=O
C(C)(=O)SCC1C(N[C@@H](CSCCCCCCC1)C(=O)O)=O.C([O-])([O-])=O.[Cs+].[Cs+].C(C1=CC=CC=C1)Br>>C(C)(=O)SCC1C(N[C@@H](CSCCCCCCC1)C(=O)OCC1=CC=CC=C1)=O
Br[CH2:20][c:21]1[cH:22][cH:23][cH:24][cH:25][cH:26]1.[CH3:1][C:2](=[O:3])[S:4][CH2:5][CH:6]1[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][CH2:13][S:14][CH2:15][C@@H:16]([C:17](=[O:18])[OH:19])[NH:27][C:28]1=[O:29]>>[CH3:1][C:2](=[O:3])[S:4][CH2:5][CH:6]1[CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][CH2:13][S:14][CH2:1...
BrCc1ccccc1.CC(=O)SCC1CCCCCCCSC[C@@H](C(=O)O)NC1=O
CC(=O)SCC1CCCCCCCSC[C@@H](C(=O)OCc2ccccc2)NC1=O
null
null
O
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
06c4f868ad4646eea8208ecb83f54ca035dd62d04f0d8101641a4f487f2c695c
8446834f0edd1e71a2dcaffc09b80c7367abf3407263a8998354a2d20c1766bb
O=C1CCCCCCCCSC[C@@H](C(=O)OCc2ccccc2)N1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[#7:5]-[C:6]-[C:7](=[O;D1;H0:8])-[OH;D1;+0:9]>>[#7:5]-[C:6]-[C:7](=[O;D1;H0:8])-[O;H0;D2;+0:9]-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
8
HOUR
(3R)-6-(Acetylthiomethyl)-5-oxo-1-thia-4-azacyclotridecane-3-carboxylic acid (0.62 g, 1.78 mmol) is dissolved in dimethylformide (8 ml) and cesium carbonate (0.64 g, 1.96 mmol) is added, followed by benzyl bromide (0.31 g, 1.78 mmol). The mixture is stirred overnight at room temperature, poured into water (300 ml) and ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Carboxylic acid
Ester
null
null
C1CCCCNCCSCCCC1.c1ccccc1
HBr
O
null
8
BrCc1ccccc1.CC(=O)SCC1CCCCCCCSC[C@@H](C(=O)O)NC1=O>O>CC(=O)SCC1CCCCCCCSC[C@@H](C(=O)OCc2ccccc2)NC1=O
ord_dataset-02ee2261663048188cf6d85d2cc96e3f
ord-f3916e44658846b1b722f56ff1174fcc
BrCc1ccccc1.CC(C)(C)C(=O)SCC1CCCCCCCSC[C@@H](C(=O)O)NC1=O>>CC(C)(C)C(=O)SCC1CCCCCCCSC[C@@H](C(=O)OCc2ccccc2)NC1=O
O.C([O-])([O-])=O.[Cs+].[Cs+].C(C(C)(C)C)(=O)SCC1C(N[C@@H](CSCCCCCCC1)C(=O)O)=O.C(C1=CC=CC=C1)Br>>C(C(C)(C)C)(=O)SCC1C(N[C@@H](CSCCCCCCC1)C(=O)OCC1=CC=CC=C1)=O
Br[CH2:23][c:24]1[cH:25][cH:26][cH:27][cH:28][cH:29]1.[CH3:1][C:2]([CH3:3])([CH3:4])[C:5](=[O:6])[S:7][CH2:8][CH:9]1[CH2:10][CH2:11][CH2:12][CH2:13][CH2:14][CH2:15][CH2:16][S:17][CH2:18][C@@H:19]([C:20](=[O:21])[OH:22])[NH:30][C:31]1=[O:32]>>[CH3:1][C:2]([CH3:3])([CH3:4])[C:5](=[O:6])[S:7][CH2:8][CH:9]1[CH2:10][CH2:11]...
BrCc1ccccc1.CC(C)(C)C(=O)SCC1CCCCCCCSC[C@@H](C(=O)O)NC1=O
CC(C)(C)C(=O)SCC1CCCCCCCSC[C@@H](C(=O)OCc2ccccc2)NC1=O
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
06c4f868ad4646eea8208ecb83f54ca035dd62d04f0d8101641a4f487f2c695c
8446834f0edd1e71a2dcaffc09b80c7367abf3407263a8998354a2d20c1766bb
O=C1CCCCCCCCSC[C@@H](C(=O)OCc2ccccc2)N1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[#7:5]-[C:6]-[C:7](=[O;D1;H0:8])-[OH;D1;+0:9]>>[#7:5]-[C:6]-[C:7](=[O;D1;H0:8])-[O;H0;D2;+0:9]-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4]
null
[]
null
null
8
HOUR
(3R)-6-(Pivaloylthiomethyl)-5-oxo-1-thia-4-azacyclotridecane-3-carboxylic acid (0.25 g, 0.64 mmol) is dissolved in dimethylformamide (5 ml) and cesium carbonate (0.23 g, 0.71 mmol) is added, followed by benzyl bromide (0.11 g, 0.64 mmol). The mixture is stirred overnight at room temperature, poured into water (300 ml) ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Carboxylic acid
Ester
null
null
C1CCCCNCCSCCCC1.c1ccccc1
HBr
CN(C=O)C
null
8
BrCc1ccccc1.CC(C)(C)C(=O)SCC1CCCCCCCSC[C@@H](C(=O)O)NC1=O>CN(C=O)C>CC(C)(C)C(=O)SCC1CCCCCCCSC[C@@H](C(=O)OCc2ccccc2)NC1=O