dataset_id
large_stringclasses
414 values
reaction_id
large_stringlengths
36
36
reaction_smiles
large_stringlengths
4
873
rxn_insight_reaction
large_stringlengths
19
1.07k
mapped_reaction_smiles
large_stringlengths
14
3.37k
reactant_smiles
large_stringlengths
1
581
product_smiles
large_stringlengths
1
433
reagent_smiles
large_stringclasses
634 values
catalyst_smiles
large_stringlengths
1
683
solvent_smiles
large_stringlengths
1
245
rxn_insight_class
large_stringclasses
11 values
rxn_insight_name
large_stringclasses
346 values
rxn_insight_tag
large_stringlengths
64
64
rxn_insight_tag2
large_stringlengths
64
64
rxn_insight_scaffold
large_stringlengths
5
288
rxn_insight_template
large_stringlengths
24
2.64k
yield_percent
float64
-0.8
90,205,160,000B
yield_measurements
large_stringlengths
2
864
temperature_value
float64
-230
30.1k
temperature_units
large_stringclasses
3 values
reaction_time_value
float64
0
4k
time_units
large_stringclasses
4 values
procedure_details
large_stringlengths
1
23.6k
reference
large_stringclasses
96 values
doi
large_stringclasses
19 values
functional_groups_reactants
large_stringlengths
3
716
functional_groups_products
large_stringlengths
3
539
participating_rings_reactants
large_stringlengths
5
293
participating_rings_products
large_stringlengths
5
271
all_rings_products
large_stringlengths
5
271
byproduct_smiles
large_stringclasses
176 values
agent_smiles
large_stringlengths
1
712
temperature_c
float64
-230
30.1k
reaction_time_hours
float64
0
2.16k
reaction_smiles_with_agents
large_stringlengths
4
882
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-cf6e582b3420469ba395e08f1c797454
Brc1nnc(-c2ccc(-c3ccccc3)nc2)n1-c1cccc2nonc12.CNCCOC>>COCCN(C)c1nnc(-c2ccc(-c3ccccc3)nc2)n1-c1cccc2nonc12
COCCNC.O.BrC1=NN=C(N1C1=CC=CC2=NON=C21)C=2C=NC(=CC2)C2=CC=CC=C2>>N=1ON=C2C1C=CC=C2N2C(=NN=C2C=2C=NC(=CC2)C2=CC=CC=C2)N(C)CCOC
Br[c:7]1[n:8][n:9][c:10](-[c:11]2[cH:12][cH:13][c:14](-[c:15]3[cH:16][cH:17][cH:18][cH:19][cH:20]3)[n:21][cH:22]2)[n:23]1-[c:24]1[cH:25][cH:26][cH:27][c:28]2[n:29][o:30][n:31][c:32]12.[CH3:1][O:2][CH2:3][CH2:4][NH:5][CH3:6]>>[CH3:1][O:2][CH2:3][CH2:4][N:5]([CH3:6])[c:7]1[n:8][n:9][c:10](-[c:11]2[cH:12][cH:13][c:14](-[c...
Brc1nnc(-c2ccc(-c3ccccc3)nc2)n1-c1cccc2nonc12.CNCCOC
COCCN(C)c1nnc(-c2ccc(-c3ccccc3)nc2)n1-c1cccc2nonc12
null
null
C(Cl)(Cl)Cl
Heteroatom Alkylation and Arylation
Ullmann-Goldberg Substitution amine
1c5140a16b98c8622dd561f15d9064ef2d9e3793a6123294dacf3a1a1e648482
b6b8e2cdb45054a35f5e8157d624f852c0601a09401556706e166b19536eb7a7
c1ccc(-c2ccc(-c3nncn3-c3cccc4nonc34)cn2)cc1
Br-[c;H0;D3;+0:1]1:[#7;a:2]:[#7;a:3]:[c:4](-[c:5]:[c:6]:[#7;a:7]):[#7;a:8]:1-[c:9]:[c:10]:[#7;a:11].[C:12]-[C:13]-[NH;D2;+0:14]-[C;D1;H3:15]>>[#7;a:7]:[c:6]:[c:5]-[c:4]1:[#7;a:3]:[#7;a:2]:[c;H0;D3;+0:1](-[N;H0;D3;+0:14](-[C;D1;H3:15])-[C:13]-[C:12]):[#7;a:8]:1-[c:9]:[c:10]:[#7;a:11]
19
[{"value": 19.0, "product": "N=1ON=C2C1C=CC=C2N2C(=NN=C2C=2C=NC(=CC2)C2=CC=CC=C2)N(C)CCOC", "details": "PERCENTYIELD", "is_desired": false}]
160
CELSIUS
6
HOUR
In a sealed tube, N-(2-methoxyethyl)methylamine (3 ml) and water (3 ml) were added to 4-[3-bromo-5-(6-phenylpyridin-3-yl)-4H-1,2,4-triazol-4-yl]-2,1,3-benzooxadiazol (336 mg) prepared in the Production Example 5, and stirred at 160° C. for 6 hours. After the reaction solution was cooled to ambient temperature, chlorofo...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Secondary amine
Tertiary amine
c1nc[nH]n1
c1nc[nH]n1
c1nc[nH]n1.c1ccncc1.c1ccccc1.c1ccc2nonc2c1
HBr
C(Cl)(Cl)Cl
160
6
Brc1nnc(-c2ccc(-c3ccccc3)nc2)n1-c1cccc2nonc12.CNCCOC>C(Cl)(Cl)Cl>COCCN(C)c1nnc(-c2ccc(-c3ccccc3)nc2)n1-c1cccc2nonc12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-815da08f3f394f2f9fe1d635be980f9a
O=C(NNC(=S)Nc1ccccc1F)c1ccc(-c2ccccc2)cc1>>Fc1ccccc1-n1c(S)nnc1-c1ccc(-c2ccccc2)cc1
C1(=CC=C(C=C1)C(=O)NNC(=S)NC1=C(C=CC=C1)F)C1=CC=CC=C1.Cl>>C1(=CC=C(C=C1)C=1N(C(=NN1)S)C1=C(C=CC=C1)F)C1=CC=CC=C1
O=[C:13]([NH:12][NH:11][C:9]([NH:8][c:7]1[c:2]([F:1])[cH:3][cH:4][cH:5][cH:6]1)=[S:10])[c:14]1[cH:15][cH:16][c:17](-[c:18]2[cH:19][cH:20][cH:21][cH:22][cH:23]2)[cH:24][cH:25]1>>[F:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1-[n:8]1[c:9]([SH:10])[n:11][n:12][c:13]1-[c:14]1[cH:15][cH:16][c:17](-[c:18]2[cH:19][cH:20][cH:21][cH:...
O=C(NNC(=S)Nc1ccccc1F)c1ccc(-c2ccccc2)cc1
Fc1ccccc1-n1c(S)nnc1-c1ccc(-c2ccccc2)cc1
null
null
[OH-].[Na+]
Aromatic Heterocycle Formation
OtherReaction
1144bd2dd2884a2ad222a26ff69bf4b180d1a69c57c6d5800b04ac08cd859d55
bd25a921a2c629db55acdd4e6573a984608495ab82bd2f024888ad689a9b3a51
c1ccc(-c2ccc(-c3nncn3-c3ccccc3)cc2)cc1
O=[C;H0;D3;+0:1](-[NH;D2;+0:2]-[NH;D2;+0:3]-[C;H0;D3;+0:4](=[S;H0;D1;+0:5])-[NH;D2;+0:6]-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10](-[F;D1;H0:11]):[c:12])-[c;H0;D3;+0:13](:[c:14]:[c:15]):[c:16]:[c:17]>>[F;D1;H0:11]-[c:10](:[c:12]):[c;H0;D3;+0:7](-[n;H0;D3;+0:6]1:[c;H0;D3;+0:1](-[c;H0;D3;+0:13](:[c:14]:[c:15]):[c:16]:[c:17]):[...
97.4
[{"value": 97.0, "product": "C1(=CC=C(C=C1)C=1N(C(=NN1)S)C1=C(C=CC=C1)F)C1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 97.4, "product": "C1(=CC=C(C=C1)C=1N(C(=NN1)S)C1=C(C=CC=C1)F)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
1-(Biphenyl-4-carbonyl)-4-(2-fluorophenyl)thiosemicarbazide (12.1 g) was suspended in aqueous 2 mol/liter sodium hydroxide solution (300 ml), and refluxed under heating for 3 hours. After the reaction solution was cooled to ambient temperature, the solution was neutralized under ice cooling with conc. hydrochloric acid...
10.6084/m9.figshare.5104873.v1
null
Acylhydrazine.Thiourea
Aromatic thiol
null
c1nnc[nH]1
c1ccccc1.c1nnc[nH]1.c1ccccc1.c1ccccc1
HO-
[OH-].[Na+]
null
null
O=C(NNC(=S)Nc1ccccc1F)c1ccc(-c2ccccc2)cc1>[OH-].[Na+]>Fc1ccccc1-n1c(S)nnc1-c1ccc(-c2ccccc2)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-ba454e8e73744cc58e8043ddd323cb9f
CI.Fc1ccccc1-n1c(S)nnc1-c1ccc(-c2ccccc2)cc1>>CSc1nnc(-c2ccc(-c3ccccc3)cc2)n1-c1ccccc1F
O.CI.C([O-])([O-])=O.[K+].[K+].C1(=CC=C(C=C1)C=1N(C(=NN1)S)C1=C(C=CC=C1)F)C1=CC=CC=C1>>C1(=CC=C(C=C1)C1=NN=C(N1C1=C(C=CC=C1)F)SC)C1=CC=CC=C1
I[CH3:1].[SH:2][c:3]1[n:4][n:5][c:6](-[c:7]2[cH:8][cH:9][c:10](-[c:11]3[cH:12][cH:13][cH:14][cH:15][cH:16]3)[cH:17][cH:18]2)[n:19]1-[c:20]1[cH:21][cH:22][cH:23][cH:24][c:25]1[F:26]>>[CH3:1][S:2][c:3]1[n:4][n:5][c:6](-[c:7]2[cH:8][cH:9][c:10](-[c:11]3[cH:12][cH:13][cH:14][cH:15][cH:16]3)[cH:17][cH:18]2)[n:19]1-[c:20]1[c...
CI.Fc1ccccc1-n1c(S)nnc1-c1ccc(-c2ccccc2)cc1
CSc1nnc(-c2ccc(-c3ccccc3)cc2)n1-c1ccccc1F
null
null
C(C)#N
Heteroatom Alkylation and Arylation
thioether_nucl_sub
cbeef1e4b9250d05ec80fbfc2f139c184e610b2c8de8aec4214044a1d69bd441
a20e50d7df818b91ffc2e826d304ad74f6246978a284c599e867e2d806b7437e
c1ccc(-c2ccc(-c3nncn3-c3ccccc3)cc2)cc1
I-[CH3;D1;+0:1].[SH;D1;+0:2]-[c:3]1:[#7;a:4]:[#7;a:5]:[c:6]:[#7;a:7]:1-[c:8]>>[CH3;D1;+0:1]-[S;H0;D2;+0:2]-[c:3]1:[#7;a:4]:[#7;a:5]:[c:6]:[#7;a:7]:1-[c:8]
72.5
[{"value": 72.0, "product": "C1(=CC=C(C=C1)C1=NN=C(N1C1=C(C=CC=C1)F)SC)C1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 72.5, "product": "C1(=CC=C(C=C1)C1=NN=C(N1C1=C(C=CC=C1)F)SC)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
5-Biphenyl-4-yl-4-(2-fluorophenyl)-4H-1,2,4-triazole-3-thiol (2.7 g) was dissolved in acetonitrile (50 ml), followed by addition of methyl iodide (0.967 ml) and potassium carbonate (1.07 g), and stirred at ambient temperature for 3 hours. Water was added to the reaction solution, followed by extraction with chloroform....
10.6084/m9.figshare.5104873.v1
null
Aromatic thiol
Monosulfide
null
null
c1nc[nH]n1.c1ccccc1.c1ccccc1.c1ccccc1
HI
C(C)#N
null
3
CI.Fc1ccccc1-n1c(S)nnc1-c1ccc(-c2ccccc2)cc1>C(C)#N>CSc1nnc(-c2ccc(-c3ccccc3)cc2)n1-c1ccccc1F
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-292a0a704b9b471094fb6636feb1e86e
Nc1ccccc1F.O=C(COCc1ccccc1)NNC(=O)c1ccc(-c2ccccc2)cc1>>Fc1ccccc1-n1c(COCc2ccccc2)nnc1-c1ccc(-c2ccccc2)cc1
C(C1=CC=CC=C1)OCC(=O)NNC(=O)C1=CC=C(C=C1)C1=CC=CC=C1.P(=O)(Cl)(Cl)Cl.FC1=C(N)C=CC=C1>>C(C1=CC=CC=C1)OCC1=NN=C(N1C1=C(C=CC=C1)F)C1=CC=C(C=C1)C1=CC=CC=C1
[F:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1[NH2:8].O=[C:9]([CH2:10][O:11][CH2:12][c:13]1[cH:14][cH:15][cH:16][cH:17][cH:18]1)[NH:19][NH:20][C:21](=O)[c:22]1[cH:23][cH:24][c:25](-[c:26]2[cH:27][cH:28][cH:29][cH:30][cH:31]2)[cH:32][cH:33]1>>[F:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1-[n:8]1[c:9]([CH2:10][O:11][CH2:12][c:13]2...
Nc1ccccc1F.O=C(COCc1ccccc1)NNC(=O)c1ccc(-c2ccccc2)cc1
Fc1ccccc1-n1c(COCc2ccccc2)nnc1-c1ccc(-c2ccccc2)cc1
null
null
C(C)(=O)OCC
Aromatic Heterocycle Formation
OtherReaction
1491874fb5fa5a2454282fe5563ef779325446dc805436f30dc5afd38438560d
1f5c57f9ffab8a5214b697412c1715772187bdfe92c542c30f8b933239b9a67f
c1ccc(COCc2nnc(-c3ccc(-c4ccccc4)cc3)n2-c2ccccc2)cc1
O=[C;H0;D3;+0:1](-[NH;D2;+0:2]-[NH;D2;+0:3]-[C;H0;D3;+0:4](=O)-[C:5]-[#8:6])-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10]:[c:11].[F;D1;H0:12]-[c:13](:[c:14]):[c;H0;D3;+0:15](-[NH2;D1;+0:16]):[c:17]:[c:18]>>[#8:6]-[C:5]-[c;H0;D3;+0:4]1:[n;H0;D2;+0:3]:[n;H0;D2;+0:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:10]:[c:11]):[n;H...
58
[{"value": 58.0, "product": "C(C1=CC=CC=C1)OCC1=NN=C(N1C1=C(C=CC=C1)F)C1=CC=C(C=C1)C1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}]
100
CELSIUS
1
HOUR
To biphenyl-4-carboxylic acid N′-(2-benzyloxyacetyl)hydrazide (9.38 g) was added phosphorus oxychloride (30 ml), and stirred at 100° C. for one hour. After the reaction solution was cooled to ambient temperature, the reaction solution was concentrated under reduced pressure. To the resulting residue was added ethyl ace...
10.6084/m9.figshare.5104873.v1
null
Acylhydrazine.Acylhydrazine.Primary amine
null
null
c1nnc[nH]1
c1ccccc1.c1ccccc1.c1nnc[nH]1.c1ccccc1.c1ccccc1
HO-
C(C)(=O)OCC
100
1
Nc1ccccc1F.O=C(COCc1ccccc1)NNC(=O)c1ccc(-c2ccccc2)cc1>C(C)(=O)OCC>Fc1ccccc1-n1c(COCc2ccccc2)nnc1-c1ccc(-c2ccccc2)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-72a613d6a0154eb18a05f5ad89f90f0a
Fc1ccccc1-n1c(COCc2ccccc2)nnc1-c1ccc(-c2ccccc2)cc1>>OCc1nnc(-c2ccc(-c3ccccc3)cc2)n1-c1ccccc1F
B(Cl)(Cl)Cl.CCCCCC.C(C1=CC=CC=C1)OCC1=NN=C(N1C1=C(C=CC=C1)F)C1=CC=C(C=C1)C1=CC=CC=C1.CO.C(O)([O-])=O.[Na+]>>C1(=CC=C(C=C1)C=1N(C(=NN1)CO)C1=C(C=CC=C1)F)C1=CC=CC=C1
c1ccc(C[O:1][CH2:2][c:3]2[n:4][n:5][c:6](-[c:7]3[cH:8][cH:9][c:10](-[c:11]4[cH:12][cH:13][cH:14][cH:15][cH:16]4)[cH:17][cH:18]3)[n:19]2-[c:20]2[cH:21][cH:22][cH:23][cH:24][c:25]2[F:26])cc1>>[OH:1][CH2:2][c:3]1[n:4][n:5][c:6](-[c:7]2[cH:8][cH:9][c:10](-[c:11]3[cH:12][cH:13][cH:14][cH:15][cH:16]3)[cH:17][cH:18]2)[n:19]1-...
Fc1ccccc1-n1c(COCc2ccccc2)nnc1-c1ccc(-c2ccccc2)cc1
OCc1nnc(-c2ccc(-c3ccccc3)cc2)n1-c1ccccc1F
null
null
C(Cl)(Cl)Cl
Deprotection
Hydroxyl benzyl deprotection
c8a6fd2e05b2d36256c76b73aaf4118f20eb14abce1c0289b554265e30b218aa
29a81fd08d26edc3da6d72c4958026f5af2119326dc1b4714ee5be1c41835609
c1ccc(-c2ccc(-c3nncn3-c3ccccc3)cc2)cc1
[#7;a:1]:[c:2](-[C:3]-[O;H0;D2;+0:4]-C-c1:c:c:c:c:c:1):[#7;a:5]:[#7;a:6]>>[#7;a:1]:[c:2](-[C:3]-[OH;D1;+0:4]):[#7;a:5]:[#7;a:6]
44
[{"value": 44.0, "product": "C1(=CC=C(C=C1)C=1N(C(=NN1)CO)C1=C(C=CC=C1)F)C1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}, {"value": 43.9, "product": "C1(=CC=C(C=C1)C=1N(C(=NN1)CO)C1=C(C=CC=C1)F)C1=CC=CC=C1", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
3-Benzyloxymethyl-5-biphenyl-4-yl-4-(2-fluorophenyl)-4H-1,2,4-triazole (6.00 g) was dissolved in chloroform (200 ml), followed by dropwise addition of 1 mol/liter boron trichloride-hexane solution (30 ml) at −44° C. and stirred at the same temperature for 30 minutes and at ambient temperature for one hour. To the react...
10.6084/m9.figshare.5104873.v1
null
Ether
Primary alcohol
c1ccccc1
null
c1nc[nH]n1.c1ccccc1.c1ccccc1.c1ccccc1
Other
C(Cl)(Cl)Cl
null
1
Fc1ccccc1-n1c(COCc2ccccc2)nnc1-c1ccc(-c2ccccc2)cc1>C(Cl)(Cl)Cl>OCc1nnc(-c2ccc(-c3ccccc3)cc2)n1-c1ccccc1F
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-6dc921bf4d444f74b81d08626569b52f
O=S(Cl)Cl.OCc1nnc(-c2ccc(-c3ccccc3)cc2)n1-c1ccccc1F>>Fc1ccccc1-n1c(CCl)nnc1-c1ccc(-c2ccccc2)cc1
C1(=CC=C(C=C1)C=1N(C(=NN1)CO)C1=C(C=CC=C1)F)C1=CC=CC=C1.S(=O)(Cl)Cl.C(Cl)(Cl)Cl>>C1(=CC=C(C=C1)C1=NN=C(N1C1=C(C=CC=C1)F)CCl)C1=CC=CC=C1
O=S(Cl)[Cl:11].O[CH2:10][c:9]1[n:8](-[c:7]2[c:2]([F:1])[cH:3][cH:4][cH:5][cH:6]2)[c:14](-[c:15]2[cH:16][cH:17][c:18](-[c:19]3[cH:20][cH:21][cH:22][cH:23][cH:24]3)[cH:25][cH:26]2)[n:13][n:12]1>>[F:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1-[n:8]1[c:9]([CH2:10][Cl:11])[n:12][n:13][c:14]1-[c:15]1[cH:16][cH:17][c:18](-[c:19]2[...
O=S(Cl)Cl.OCc1nnc(-c2ccc(-c3ccccc3)cc2)n1-c1ccccc1F
Fc1ccccc1-n1c(CCl)nnc1-c1ccc(-c2ccccc2)cc1
null
null
C1(=CC=CC=C1)C
Functional Group Interconversion
Alcohol to chloride_SOCl2
bb752b9027dc4488ba075e5955118a819f80cabd751a7497b67c2eeb1db6b071
cbf41c7cf9fe6b47a243b1674d74ed5bf46a151f7f3a71d206e23176e158facf
c1ccc(-c2ccc(-c3nncn3-c3ccccc3)cc2)cc1
Cl-S(=O)-[Cl;H0;D1;+0:1].O-[CH2;D2;+0:2]-[c:3]1:[#7;a:4]:[#7;a:5]:[c:6]:[#7;a:7]:1-[c:8]>>[Cl;H0;D1;+0:1]-[CH2;D2;+0:2]-[c:3]1:[#7;a:4]:[#7;a:5]:[c:6]:[#7;a:7]:1-[c:8]
81
[{"value": 81.0, "product": "C1(=CC=C(C=C1)C1=NN=C(N1C1=C(C=CC=C1)F)CCl)C1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}]
60
CELSIUS
5
HOUR
[5-Biphenyl-4-yl-4-(2-fluorophenyl)-4H-1,2,4-triazol-3-yl]methanol (1.81 g) was suspended in toluene (25 ml), followed by addition of thionyl chloride (1.5 ml) and chloroform (25 ml), and stirred at 60° C. for 5 hours. After the reaction solution was concentrated under reduced pressure, ethyl acetate was added to the r...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol
Primary halide
null
null
c1ccccc1.c1nnc[nH]1.c1ccccc1.c1ccccc1
HCl
C1(=CC=CC=C1)C
60
5
O=S(Cl)Cl.OCc1nnc(-c2ccc(-c3ccccc3)cc2)n1-c1ccccc1F>C1(=CC=CC=C1)C>Fc1ccccc1-n1c(CCl)nnc1-c1ccc(-c2ccccc2)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-7794f3c01c4a42198c2584e503f849f8
C1COCCN1.Fc1ccccc1-n1c(CCl)nnc1-c1ccc(-c2ccccc2)cc1>>Fc1ccccc1-n1c(CN2CCOCC2)nnc1-c1ccc(-c2ccccc2)cc1
N1CCOCC1.[H-].[Na+].C1(=CC=C(C=C1)C1=NN=C(N1C1=C(C=CC=C1)F)CCl)C1=CC=CC=C1>>C1(=CC=C(C=C1)C=1N(C(=NN1)CN1CCOCC1)C1=C(C=CC=C1)F)C1=CC=CC=C1
[NH:11]1[CH2:12][CH2:13][O:14][CH2:15][CH2:16]1.Cl[CH2:10][c:9]1[n:8](-[c:7]2[c:2]([F:1])[cH:3][cH:4][cH:5][cH:6]2)[c:19](-[c:20]2[cH:21][cH:22][c:23](-[c:24]3[cH:25][cH:26][cH:27][cH:28][cH:29]3)[cH:30][cH:31]2)[n:18][n:17]1>>[F:1][c:2]1[cH:3][cH:4][cH:5][cH:6][c:7]1-[n:8]1[c:9]([CH2:10][N:11]2[CH2:12][CH2:13][O:14][C...
C1COCCN1.Fc1ccccc1-n1c(CCl)nnc1-c1ccc(-c2ccccc2)cc1
Fc1ccccc1-n1c(CN2CCOCC2)nnc1-c1ccc(-c2ccccc2)cc1
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
2bad30dcdb0a20edb8ce877f072b133eedfd870621da393ec393128bfee00977
523d37155b42c8dc851abeddadebb241cdd90bdf649ba750c35e13c8c752d7b0
c1ccc(-c2ccc(-c3nnc(CN4CCOCC4)n3-c3ccccc3)cc2)cc1
Cl-[CH2;D2;+0:1]-[c:2]1:[#7;a:3]:[#7;a:4]:[c:5]:[#7;a:6]:1-[c:7].[#8:8]1-[C:9]-[C:10]-[NH;D2;+0:11]-[C:12]-[C:13]-1>>[c:7]-[#7;a:6]1:[c:5]:[#7;a:4]:[#7;a:3]:[c:2]:1-[CH2;D2;+0:1]-[N;H0;D3;+0:11]1-[C:10]-[C:9]-[#8:8]-[C:13]-[C:12]-1
74
[{"value": 74.0, "product": "C1(=CC=C(C=C1)C=1N(C(=NN1)CN1CCOCC1)C1=C(C=CC=C1)F)C1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
Morpholine (0.599 ml) was dissolved in N,N-dimethylformamide (6 ml), followed by addition of sodium hydride (60%, 275 mg) under ice cooling, and stirred at the same temperature for 30 minutes. Under ice cooling, 3-biphenyl-4-yl-5-chloromethyl-4-(2-fluorophenyl)-4H-1,2,4-triazole (599 mg) was added to the reaction solut...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amine
Tertiary amine
C1COCCN1
C1COCC[NH]1
c1ccccc1.C1COCC[NH]1.c1nnc[nH]1.c1ccccc1.c1ccccc1
HCl
CN(C=O)C
null
0.5
C1COCCN1.Fc1ccccc1-n1c(CCl)nnc1-c1ccc(-c2ccccc2)cc1>CN(C=O)C>Fc1ccccc1-n1c(CN2CCOCC2)nnc1-c1ccc(-c2ccccc2)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-eede2b3d64ad403cbc6219dd7b894bcc
COC1CCCO1.c1cnc2[nH]ccc2c1>>OCCCC(c1c[nH]c2ncccc12)c1c[nH]c2ncccc12
N1C=CC2=CC=CN=C12.COC1OCCC1>>N1C=C(C2=CC=CN=C12)C(CCCO)C1=CNC2=NC=CC=C12
O([CH:5]1[O:1][CH2:2][CH2:3][CH2:4]1)[CH3:11].[cH:6]1[cH:7][nH:8][c:9]2[c:14]1[cH:13][cH:12][cH:20][n:19]2>>[OH:1][CH2:2][CH2:3][CH2:4][CH:5]([c:6]1[cH:7][nH:8][c:9]2[n:10][cH:11][cH:12][cH:13][c:14]12)[c:15]1[cH:16][nH:17][c:18]2[n:19][cH:20][cH:21][cH:22][c:23]12
COC1CCCO1.c1cnc2[nH]ccc2c1
OCCCC(c1c[nH]c2ncccc12)c1c[nH]c2ncccc12
null
null
null
Aromatic Heterocycle Formation
OtherReaction
60739617603a0725721d97ef4dccb686c3e557f71265e15aa108cdeb9d4a01ff
f4039f6137c58f023c0dcbef20c5fb1b1eb5a4818bb4583d7316df6dacf02876
c1cnc2[nH]cc(Cc3c[nH]c4ncccc34)c2c1
[#7;a:1]1:[c:2]:[cH;D2;+0:3]:[c:4]2:[c:5]:[cH;D2;+0:6]:[cH;D2;+0:7]:[n;H0;D2;+0:8]:[c;H0;D3;+0:9]:1:2.[CH3;D1;+0:10]-O-[CH;D3;+0:11]1-[C:12]-[C:13]-[C:14]-[O;H0;D2;+0:15]-1>>[OH;D1;+0:15]-[C:14]-[C:13]-[C:12]-[CH;D3;+0:11](-[c:16]1:[c:17]:[#7;a:18]:[c:19]2:[n;H0;D2;+0:8]:[cH;D2;+0:7]:[c:20]:[c:21]:[c:22]:1:2)-[c;H0;D3;...
null
[]
null
null
null
null
This compound is prepared in the same way as described in example 1/1 starting from 7-azaindol and 2-methoxy-tetrahydrofuran. Conditions: See reaction.notes.procedure_details. Workup: This compound is prepared in the same way
10.6084/m9.figshare.5104873.v1
null
Ether.Ether
Primary alcohol
C1CCOC1.c1cnc2[nH]ccc2c1
c1cnc2[nH]ccc2c1.c1cnc2[nH]ccc2c1
c1cnc2[nH]ccc2c1.c1cnc2[nH]ccc2c1
null
null
null
null
COC1CCCO1.c1cnc2[nH]ccc2c1>>OCCCC(c1c[nH]c2ncccc12)c1c[nH]c2ncccc12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-a7069c89951542c6aac014e0ba0b4104
CCCC=O.c1ccc2[nH]ccc2c1>>CCCC(c1c[nH]c2ccccc12)c1c[nH]c2ccccc12
N1C=CC2=CC=CC=C12.C(CCC)=O>>N1C=C(C2=CC=CC=C12)C(CCC)C1=CNC2=CC=CC=C12
O=[CH:4][CH2:3][CH2:2][CH3:1].[cH:5]1[cH:6][nH:7][c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]12>>[CH3:1][CH2:2][CH2:3][CH:4]([c:5]1[cH:6][nH:7][c:8]2[cH:9][cH:10][cH:11][cH:12][c:13]12)[c:14]1[cH:15][nH:16][c:17]2[cH:18][cH:19][cH:20][cH:21][c:22]12
CCCC=O.c1ccc2[nH]ccc2c1
CCCC(c1c[nH]c2ccccc12)c1c[nH]c2ccccc12
null
null
CO.O
Aromatic Heterocycle Formation
OtherReaction
7478ef73472b362e627cc75f333e4944966fb671972736fb7b88535ca746eb04
208b563f3abf251ea7444c9cd3c4f06a2ed6563578ed1cbc46d48e2aa059bd9b
c1ccc2c(Cc3c[nH]c4ccccc34)c[nH]c2c1
O=[CH;D2;+0:1]-[C:2]-[C:3].[c:4]:[c:5]1:[cH;D2;+0:6]:[c:7]:[#7;a:8]:[c:9]:1:[c:10]>>[C:3]-[C:2]-[CH;D3;+0:1](-[c:11](:[c:12]):[c:13])-[c;H0;D3;+0:6]1:[c:7]:[#7;a:8]:[c:9](:[c:10]):[c:5]:1:[c:4]
null
[]
null
null
null
null
282 mg of indole (2.4 mmol) were dissolved in 10 ml of CH3OH and 5 ml of H2O; 72 mg (1 mmol) of butyraldehyde and 240 mg of dysprosium triflate-(CF3SO3)3Dy-(0.393 mmol) were added. Conditions: See reaction.notes.procedure_details.
10.6084/m9.figshare.5104873.v1
null
Aldehyde
null
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.c1ccc2[nH]ccc2c1
null
CO.O
null
null
CCCC=O.c1ccc2[nH]ccc2c1>CO.O>CCCC(c1c[nH]c2ccccc12)c1c[nH]c2ccccc12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-f5f5a80157ad4bdca616f4b651e2eecb
CCCC=O.O=[N+]([O-])c1ccc2[nH]ccc2c1>>CCCC(c1c[nH]c2ccc([N+](=O)[O-])cc12)c1c[nH]c2ccc([N+](=O)[O-])cc12
[N+](=O)([O-])C=1C=C2C=CNC2=CC1.C(CCC)=O>>[N+](=O)([O-])C=1C=C2C(=CNC2=CC1)C(CCC)C1=CNC2=CC=C(C=C12)[N+](=O)[O-]
[CH3:1][CH2:2][CH2:3][CH:4]=[O:13].[cH:5]1[cH:6][nH:7][c:8]2[cH:9][cH:10][c:23]([N+:24]([O-:14])=[O:25])[cH:27][c:16]12>>[CH3:1][CH2:2][CH2:3][CH:4]([c:5]1[cH:6][nH:7][c:8]2[cH:9][cH:10][c:11]([N+:12](=[O:13])[O-:14])[cH:15][c:16]12)[c:17]1[cH:18][nH:19][c:20]2[cH:21][cH:22][c:23]([N+:24](=[O:25])[O-:26])[cH:27][c:28]1...
CCCC=O.O=[N+]([O-])c1ccc2[nH]ccc2c1
CCCC(c1c[nH]c2ccc([N+](=O)[O-])cc12)c1c[nH]c2ccc([N+](=O)[O-])cc12
null
null
null
Aromatic Heterocycle Formation
OtherReaction
02371de143030bb6675629fd0d2b1da4e29d09cf183a8777e6aa524bfe2352b9
c192aaf31db94f00670e2c5a2d22e644d14ddc3b1ea4f4f1f58ffb114905b5a5
c1ccc2c(Cc3c[nH]c4ccccc34)c[nH]c2c1
[C:1]-[C:2]-[CH;D2;+0:3]=[O;H0;D1;+0:4].[O-;H0;D1:5]-[N+;H0;D3:6](=[O;D1;H0:7])-[c;H0;D3;+0:8]1:[cH;D2;+0:9]:[c:10]:[c:11]2:[#7;a:12]:[c:13]:[cH;D2;+0:14]:[c;H0;D3;+0:15]:2:[cH;D2;+0:16]:1>>[C:1]-[C:2]-[CH;D3;+0:3](-[c:17](:[c:18]):[c:19]1:[c:20]:[c:21]:[c:22]:[c;H0;D3;+0:8](-[N+;H0;D3:6](-[O;-;D1;H0:23])=[O;D1;H0:7]):...
null
[]
null
null
null
null
ST 1429 was prepared from 5-nitroindole and butyraldehyde prepared using the method described in example 2/1. Conditions: See reaction.notes.procedure_details. Workup: prepared
10.6084/m9.figshare.5104873.v1
null
Aldehyde.Nitro group
Nitro group.Nitro group
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.c1ccc2[nH]ccc2c1
Other
null
null
null
CCCC=O.O=[N+]([O-])c1ccc2[nH]ccc2c1>>CCCC(c1c[nH]c2ccc([N+](=O)[O-])cc12)c1c[nH]c2ccc([N+](=O)[O-])cc12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-40492c21a69f46b88fd0fa2d519864ca
CCCC=O.Fc1ccc2[nH]ccc2c1>>CCCC(c1c[nH]c2ccc(F)cc12)c1c[nH]c2ccc(F)cc12
FC=1C=C2C=CNC2=CC1.C(CCC)=O>>FC=1C=C2C(=CNC2=CC1)C(CCC)C1=CNC2=CC=C(C=C12)F
O=[CH:4][CH2:3][CH2:2][CH3:1].[cH:5]1[cH:6][nH:7][c:8]2[cH:9][cH:10][c:11]([F:12])[cH:13][c:14]12>>[CH3:1][CH2:2][CH2:3][CH:4]([c:5]1[cH:6][nH:7][c:8]2[cH:9][cH:10][c:11]([F:12])[cH:13][c:14]12)[c:15]1[cH:16][nH:17][c:18]2[cH:19][cH:20][c:21]([F:22])[cH:23][c:24]12
CCCC=O.Fc1ccc2[nH]ccc2c1
CCCC(c1c[nH]c2ccc(F)cc12)c1c[nH]c2ccc(F)cc12
null
null
null
Aromatic Heterocycle Formation
OtherReaction
ec460e45d4b7f4f683438c9409b11235f5dae08ccdc80957cd49fe1fd35b87d0
31aeef82055455d7a38ad7be94e5da21cccc4998cb40f7eea686b19a2150757f
c1ccc2c(Cc3c[nH]c4ccccc34)c[nH]c2c1
O=[CH;D2;+0:1]-[C:2]-[C:3].[c:4]:[c:5]1:[cH;D2;+0:6]:[c:7]:[#7;a:8]:[c:9]:1:[c:10]>>[C:3]-[C:2]-[CH;D3;+0:1](-[c:11](:[c:12]):[c:13])-[c;H0;D3;+0:6]1:[c:7]:[#7;a:8]:[c:9](:[c:10]):[c:5]:1:[c:4]
45
[{"value": 45.0, "product": "FC=1C=C2C(=CNC2=CC1)C(CCC)C1=CNC2=CC=C(C=C12)F", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This was prepared in the same way as described in example 2/2 starting from 5-fluoroindole and butyraldehyde. The reaction, however, was heated under reflux for 24 hours. The end product was isolated and purified by chromatography on an SiO2 column using a hexane:ethyl ether gradient ranging from 7:3 to 4:6 as the elue...
10.6084/m9.figshare.5104873.v1
null
Aldehyde
Aromatic halide
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.c1ccc2[nH]ccc2c1
null
null
null
null
CCCC=O.Fc1ccc2[nH]ccc2c1>>CCCC(c1c[nH]c2ccc(F)cc12)c1c[nH]c2ccc(F)cc12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-7e699b14c36a4cb1ab9bfad78d80f704
CCCC=O.c1cnc2[nH]ccc2c1>>CCCC(c1c[nH]c2ncccc12)c1c[nH]c2ncccc12
N1C=CC2=CC=CN=C12.C(CCC)=O>>N1C=C(C2=CC=CN=C12)C(CCC)C1=CNC2=NC=CC=C12
O=[CH:4][CH2:3][CH2:2][CH3:1].[cH:5]1[cH:6][nH:7][c:8]2[c:13]1[cH:12][cH:11][cH:19][n:18]2>>[CH3:1][CH2:2][CH2:3][CH:4]([c:5]1[cH:6][nH:7][c:8]2[n:9][cH:10][cH:11][cH:12][c:13]12)[c:14]1[cH:15][nH:16][c:17]2[n:18][cH:19][cH:20][cH:21][c:22]12
CCCC=O.c1cnc2[nH]ccc2c1
CCCC(c1c[nH]c2ncccc12)c1c[nH]c2ncccc12
null
null
null
Aromatic Heterocycle Formation
OtherReaction
808e4420e445f28e4eb1512fcdbecfad15d93171379a5ec564a53c5e21e27a6b
208b563f3abf251ea7444c9cd3c4f06a2ed6563578ed1cbc46d48e2aa059bd9b
c1cnc2[nH]cc(Cc3c[nH]c4ncccc34)c2c1
O=[CH;D2;+0:1]-[C:2]-[C:3].[#7;a:4]1:[c:5]:[cH;D2;+0:6]:[c:7]2:[c:8]:[cH;D2;+0:9]:[cH;D2;+0:10]:[n;H0;D2;+0:11]:[c;H0;D3;+0:12]:1:2>>[C:3]-[C:2]-[CH;D3;+0:1](-[c:13]1:[c:14]:[#7;a:15]:[c:16]2:[n;H0;D2;+0:11]:[cH;D2;+0:10]:[c:17]:[c:18]:[c:19]:1:2)-[c;H0;D3;+0:6]1:[c:5]:[#7;a:4]:[c;H0;D3;+0:12]2:[#7;a:20]:[c:21]:[cH;D2;...
15
[{"value": 15.0, "product": "N1C=C(C2=CC=CN=C12)C(CCC)C1=CNC2=NC=CC=C12", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
ST 1436 was prepared as described in example 2/2 from 7-azaindole and butyraldehyde. The reaction, however, was heated under reflux for 48 hours. The end product was isolated and purified chromatographically on a silica column eluting with a CH2Cl2:CH3COCH3 gradient ranging from 9:1 to 4:6. Yield 15%. Conditions: See r...
10.6084/m9.figshare.5104873.v1
null
Aldehyde
null
c1cnc2[nH]ccc2c1
c1cnc2[nH]ccc2c1.c1cnc2[nH]ccc2c1
c1cnc2[nH]ccc2c1.c1cnc2[nH]ccc2c1
null
null
null
null
CCCC=O.c1cnc2[nH]ccc2c1>>CCCC(c1c[nH]c2ncccc12)c1c[nH]c2ncccc12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-04e0ea007ddc44a8939ea2cef695c555
CCCCCCCCCCCCCC=O.c1ccc2[nH]ccc2c1>>CCCCCCCCCCCCCC(c1c[nH]c2ccccc12)c1c[nH]c2ccccc12
N1C=CC2=CC=CC=C12.C(CCCCCCCCCCCCC)=O>>N1C=C(C2=CC=CC=C12)C(CCCCCCCCCCCCC)C1=CNC2=CC=CC=C12
O=[CH:25][CH2:24][CH2:14][CH2:13][CH2:12][CH2:11][CH2:10][CH2:9][CH2:8][CH2:7][CH2:6][CH2:5][CH2:4][CH3:1].[cH:15]1[cH:16][nH:17][c:18]2[cH:19][cH:20][cH:21][cH:22][c:23]12>>[CH3:1][CH2:2][CH2:3][CH2:4][CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][CH2:11][CH2:12][CH2:13][CH:14]([c:15]1[cH:16][nH:17][c:18]2[cH:19][cH:20][...
CCCCCCCCCCCCCC=O.c1ccc2[nH]ccc2c1
CCCCCCCCCCCCCC(c1c[nH]c2ccccc12)c1c[nH]c2ccccc12
null
null
null
Aromatic Heterocycle Formation
OtherReaction
7478ef73472b362e627cc75f333e4944966fb671972736fb7b88535ca746eb04
208b563f3abf251ea7444c9cd3c4f06a2ed6563578ed1cbc46d48e2aa059bd9b
c1ccc2c(Cc3c[nH]c4ccccc34)c[nH]c2c1
O=[CH;D2;+0:1]-[CH2;D2;+0:2]-[CH2;D2;+0:3]-[C:4]-[C:5].[C:6]-[C:7]-[CH2;D2;+0:8]-[CH3;D1;+0:9].[c:10]:[c:11]1:[#7;a:12]:[c:13]:[cH;D2;+0:14]:[c:15]:1:[c:16]>>[C:6]-[C:7]-[CH2;D2;+0:8]-[C:17]-[C:18]-[CH3;D1;+0:9].[C:5]-[C:4]-[CH;D3;+0:3](-[c;H0;D3;+0:14]1:[c:13]:[#7;a:12]:[c:11](:[c:10]):[c:15]:1:[c:16])-[c;H0;D3;+0:2]1...
80
[{"value": 80.0, "product": "N1C=C(C2=CC=CC=C12)C(CCCCCCCCCCCCC)C1=CNC2=CC=CC=C12", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The compound was prepared as described in example 2/4, reacting the indole with tetradecane aldehyde. Yield 80%. Conditions: See reaction.notes.procedure_details. Workup: The compound was prepared
10.6084/m9.figshare.5104873.v1
null
Aldehyde
null
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.c1ccc2[nH]ccc2c1
null
null
null
null
CCCCCCCCCCCCCC=O.c1ccc2[nH]ccc2c1>>CCCCCCCCCCCCCC(c1c[nH]c2ccccc12)c1c[nH]c2ccccc12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-34ed5aa2890246b9ad2d8473b2804b63
CCCC=O.c1cc[nH]c1>>CCCC(c1ccc[nH]1)c1ccc[nH]1
N1C=CC=C1.C(CCC)=O>>N1C(=CC=C1)C(CCC)C=1NC=CC1
O=[CH:4][CH2:3][CH2:2][CH3:1].[cH:5]1[cH:6][cH:7][cH:8][nH:9]1>>[CH3:1][CH2:2][CH2:3][CH:4]([c:5]1[cH:6][cH:7][cH:8][nH:9]1)[c:10]1[cH:11][cH:12][cH:13][nH:14]1
CCCC=O.c1cc[nH]c1
CCCC(c1ccc[nH]1)c1ccc[nH]1
null
null
null
Aromatic Heterocycle Formation
OtherReaction
b732ccc2ebe5ae50bce53fc187224a141e12227e8b603f4b5e25f82a4de1cafe
208b563f3abf251ea7444c9cd3c4f06a2ed6563578ed1cbc46d48e2aa059bd9b
c1c[nH]c(Cc2ccc[nH]2)c1
O=[CH;D2;+0:1]-[C:2]-[C:3].[#7;a:4]1:[c:5]:[c:6]:[c:7]:[cH;D2;+0:8]:1>>[#7;a:9]:[c:10](-[CH;D3;+0:1](-[C:2]-[C:3])-[c;H0;D3;+0:8]1:[#7;a:4]:[c:5]:[c:6]:[c:7]:1):[c:11]
45
[{"value": 45.0, "product": "N1C(=CC=C1)C(CCC)C=1NC=CC1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
This was prepared as described in example 2/4, reacting the pyrrole derivative with butyraldehyde. Yield 45%. Conditions: See reaction.notes.procedure_details. Workup: This was prepared
10.6084/m9.figshare.5104873.v1
null
Aldehyde
null
c1cc[nH]c1
c1cc[nH]c1.c1cc[nH]c1
c1cc[nH]c1.c1cc[nH]c1
null
null
null
null
CCCC=O.c1cc[nH]c1>>CCCC(c1ccc[nH]1)c1ccc[nH]1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-ce562329315947d4a7330023ab1ce86c
O.c1ccc2[nH]ccc2c1>>O=C(O)CCC(n1ccc2ccccc21)n1ccc2ccccc21
O.N1C=CC2=CC=CC=C12>>N1(C=CC2=CC=CC=C12)C(CCC(=O)O)N1C=CC2=CC=CC=C12
[OH2:1].[cH:2]1[cH:11][c:10]2[cH:9][cH:8][nH:7][c:15]2[cH:14][cH:13]1>>[O:1]=[C:2]([OH:3])[CH2:4][CH2:5][CH:6]([n:7]1[cH:8][cH:9][c:10]2[cH:11][cH:12][cH:13][cH:14][c:15]12)[n:16]1[cH:17][cH:18][c:19]2[cH:20][cH:21][cH:22][cH:23][c:24]12
O.c1ccc2[nH]ccc2c1
O=C(O)CCC(n1ccc2ccccc21)n1ccc2ccccc21
null
null
CO
Aromatic Heterocycle Formation
OtherReaction
be0a6a5708f4255fc1dc22abadb70851316780d90ed7242acaafd2618f261df5
9c7315ed19eeb7fef800780efa97a4613aacc14e062139968377b759809e441c
c1ccc2c(c1)ccn2Cn1ccc2ccccc21
[OH2;D0;+0:1].[c:2]1:[cH;D2;+0:3]:[cH;D2;+0:4]:[cH;D2;+0:5]:[c:6]2:[c:7]:[c:8]:[nH;D2;+0:9]:[c:10]:1:2>>[#7;a:11]-[C:12](-[C:13]-[C:14]-[C;H0;D3;+0:4](-[O;D1;H1:15])=[O;H0;D1;+0:1])-[n;H0;D3;+0:9]1:[c:8]:[c:7]:[c:6]2:[cH;D2;+0:5]:[c:16]:[cH;D2;+0:3]:[c:2]:[c:10]:2:1
null
[]
35
CELSIUS
24
HOUR
282 mg of indole (2.4 mmol) were dissolved in 10 ml of CH3OH and 5 ml of H2O; 102 mg of semisuccinic aldehyde (1 mmol) and 240 mg of dysprosium triflate-(CF3SO3)3Dy-(0.393 mmol) were added. The resulting solution was stirred at 35° C. for 24 hours. At the end of that period the methanol was removed under vacuum and the...
10.6084/m9.figshare.5104873.v1
null
null
Carboxylic acid
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.c1ccc2[nH]ccc2c1
Other
CO
35
24
O.c1ccc2[nH]ccc2c1>CO>O=C(O)CCC(n1ccc2ccccc21)n1ccc2ccccc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-21f8ef08222e47529862c9541bf0a48e
COC1CCCO1.c1ccc2[nH]ccc2c1>>OCCCC(c1c[nH]c2ccccc12)c1c[nH]c2ccccc12
N1C=CC2=CC=CC=C12.COC1OCCC1>>N1C=C(C2=CC=CC=C12)C(CCCO)C1=CNC2=CC=CC=C12
O1[CH:18]([O:1][CH3:2])[CH2:19][CH2:20][CH2:21]1.[cH:6]1[cH:7][nH:8][c:9]2[cH:10][cH:11][cH:12][cH:13][c:14]12>>[OH:1][CH2:2][CH2:3][CH2:4][CH:5]([c:6]1[cH:7][nH:8][c:9]2[cH:10][cH:11][cH:12][cH:13][c:14]12)[c:15]1[cH:16][nH:17][c:18]2[cH:19][cH:20][cH:21][cH:22][c:23]12
COC1CCCO1.c1ccc2[nH]ccc2c1
OCCCC(c1c[nH]c2ccccc12)c1c[nH]c2ccccc12
null
null
null
Aromatic Heterocycle Formation
OtherReaction
0579d4344dbff33158f2416531f0c0c5490807d596e12ff564f95d1492238351
f4039f6137c58f023c0dcbef20c5fb1b1eb5a4818bb4583d7316df6dacf02876
c1ccc2c(Cc3c[nH]c4ccccc34)c[nH]c2c1
[CH3;D1;+0:1]-[O;H0;D2;+0:2]-[CH;D3;+0:3]1-O-[CH2;D2;+0:4]-[CH2;D2;+0:5]-[CH2;D2;+0:6]-1.[c:7]:[c:8]1:[#7;a:9]:[c:10]:[cH;D2;+0:11]:[c:12]:1:[c:13]>>[OH;D1;+0:2]-[CH2;D2;+0:1]-[C:14]-[C:15]-[C:16](-[c:17]1:[c:18]:[#7;a:19]:[c;H0;D3;+0:3]2:[cH;D2;+0:6]:[cH;D2;+0:5]:[cH;D2;+0:4]:[c:20]:[c:21]:1:2)-[c;H0;D3;+0:11]1:[c:10]...
null
[]
null
null
null
null
The compound was prepared in the same way as described in example 2/4, starting from indole and 2-methoxy-tetrahydrofuran. Conditions: See reaction.notes.procedure_details. Workup: The compound was prepared in the same way
10.6084/m9.figshare.5104873.v1
null
Ether.Ether
Primary alcohol
C1CCOC1.c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.c1ccc2[nH]ccc2c1
null
null
null
null
COC1CCCO1.c1ccc2[nH]ccc2c1>>OCCCC(c1c[nH]c2ccccc12)c1c[nH]c2ccccc12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-4dd0bc4fe8c64d9e8f8801e446e2f232
CCCC(c1c[nH]c2ccccc12)c1c[nH]c2ccccc12.ClCc1ccccc1>>CCCC(c1cn(Cc2ccccc2)c2ccccc12)c1cn(Cc2ccccc2)c2ccccc12
N1C=C(C2=CC=CC=C12)C(CCC)C1=CNC2=CC=CC=C12.C(C1=CC=CC=C1)Cl>>C(C1=CC=CC=C1)N1C=C(C2=CC=CC=C12)C(CCC)C1=CN(C2=CC=CC=C12)CC1=CC=CC=C1
[CH3:1][CH2:2][CH2:3][CH:4]([c:5]1[cH:6][nH:7][c:15]2[cH:16][cH:17][cH:18][cH:19][c:20]12)[c:21]1[cH:22][nH:23][c:31]2[cH:32][cH:8][cH:34][cH:35][c:36]12.Cl[CH2:24][c:25]1[cH:26][cH:27][cH:28][cH:29][cH:30]1>>[CH3:1][CH2:2][CH2:3][CH:4]([c:5]1[cH:6][n:7]([CH2:8][c:9]2[cH:10][cH:11][cH:12][cH:13][cH:14]2)[c:15]2[cH:16][...
CCCC(c1c[nH]c2ccccc12)c1c[nH]c2ccccc12.ClCc1ccccc1
CCCC(c1cn(Cc2ccccc2)c2ccccc12)c1cn(Cc2ccccc2)c2ccccc12
null
[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC
O.C(Cl)(Cl)Cl
Aromatic Heterocycle Formation
OtherReaction
a81b71b4c4c3b573719981f1d2cd0559bc3698c6db2b57a3252a026744953a32
bba2945f18bbb88e48f2c5641704d2237fa5a07400e9b29e8d58901a4d971dcb
c1ccc(Cn2cc(Cc3cn(Cc4ccccc4)c4ccccc34)c3ccccc32)cc1
Cl-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[c:5]1:[c:6]:[nH;D2;+0:7]:[c:8]2:[cH;D2;+0:9]:[cH;D2;+0:10]:[cH;D2;+0:11]:[c:12]:[c:13]:1:2.[c:14]:[c:15]1:[c:16]:[c:17]:[c:18]:[nH;D2;+0:19]:1>>[c:3]:[c:2](-[CH2;D2;+0:1]-[n;H0;D3;+0:7]1:[c:6]:[c:5]:[c:13]2:[c:12]:[cH;D2;+0:11]:[c:20]:[cH;D2;+0:9]:[c:8]:2:1):[c:4].[c:21]:[c:22](-[C...
78
[{"value": 78.0, "product": "C(C1=CC=CC=C1)N1C=C(C2=CC=CC=C12)C(CCC)C1=CN(C2=CC=CC=C12)CC1=CC=CC=C1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
ST 1385 1,1-di-indol-3-yl-butane, 290 mg (1 mmol), was thoroughly mixed and blended with potassium tertbutylate (280 mg) and tetrabutylammonium bromide (20 mg). The mixture thus obtained was held under ultrasonic stirring at ambient temperature. 640 mg (5 mmol) of benzylchloride at 0° C. were then added and the ultraso...
10.6084/m9.figshare.5104873.v1
null
Primary halide
null
c1ccc2[nH]ccc2c1.c1ccc2[nH]ccc2c1
c1ccccc1.c1c[nH]c2ccccc12.c1c[nH]c2ccccc12
c1ccccc1.c1c[nH]c2ccccc12.c1ccccc1.c1c[nH]c2ccccc12
null
[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC.O.C(Cl)(Cl)Cl
null
2
CCCC(c1c[nH]c2ccccc12)c1c[nH]c2ccccc12.ClCc1ccccc1>[Br-].C(CCC)[N+](CCCC)(CCCC)CCCC.O.C(Cl)(Cl)Cl>CCCC(c1cn(Cc2ccccc2)c2ccccc12)c1cn(Cc2ccccc2)c2ccccc12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-053aef3bb4e14e958a06b1ca6a830675
Cc1cccc(O)c1[N+](=O)[O-].ClCCN1CCCC1>>Cc1cccc(OCCN2CCCC2)c1[N+](=O)[O-]
Cl.ClCCN1CCCC1.C([O-])([O-])=O.[K+].[K+].[I-].[Na+].CC=1C(=C(C=CC1)O)[N+](=O)[O-].Cl.ClCCN1CCCC1.C([O-])([O-])=O.[K+].[K+]>>CC=1C(=C(OCCN2CCCC2)C=CC1)[N+](=O)[O-]
[CH3:1][c:2]1[cH:3][cH:4][cH:5][c:6]([OH:7])[c:15]1[N+:16](=[O:17])[O-:18].Cl[CH2:8][CH2:9][N:10]1[CH2:11][CH2:12][CH2:13][CH2:14]1>>[CH3:1][c:2]1[cH:3][cH:4][cH:5][c:6]([O:7][CH2:8][CH2:9][N:10]2[CH2:11][CH2:12][CH2:13][CH2:14]2)[c:15]1[N+:16](=[O:17])[O-:18]
Cc1cccc(O)c1[N+](=O)[O-].ClCCN1CCCC1
Cc1cccc(OCCN2CCCC2)c1[N+](=O)[O-]
null
null
null
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
7e1040116e3a4cf0e8ec5cc7865388d9cd0efabce6d320a1c25a36e411018d8b
d5f4610d46ccc0478471c5bc0fb862644eaf764bbc5d93badb39d54f6ec8e0a5
c1ccc(OCCN2CCCC2)cc1
Cl-[CH2;D2;+0:1]-[C:2]-[#7:3].[OH;D1;+0:4]-[c:5](:[c:6]):[c:7]>>[#7:3]-[C:2]-[CH2;D2;+0:1]-[O;H0;D2;+0:4]-[c:5](:[c:6]):[c:7]
69
[{"value": 69.0, "product": "CC=1C(=C(OCCN2CCCC2)C=CC1)[N+](=O)[O-]", "details": "PERCENTYIELD", "is_desired": false}, {"value": 63.0, "product": "CC=1C(=C(OCCN2CCCC2)C=CC1)[N+](=O)[O-]", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
Potassium carbonate (34.9 g., 252 mmol) and sodium iodide (1.0 g., 6.5 mmol) were added to a solution of 3-methyl-2-nitrophenol (10 g., 65.3 mmol). With stirring, 1-(2-chloroethyl)-pyrrolidine hydrochloride (16.65 g., 98 mmol) was added portion-wise to the solution. The reaction mixture was refluxed for 15 hours, at wh...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic alcohol
Ether
null
null
c1ccccc1.C1CC[NH]C1
HCl
null
null
null
Cc1cccc(O)c1[N+](=O)[O-].ClCCN1CCCC1>>Cc1cccc(OCCN2CCCC2)c1[N+](=O)[O-]
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-d630b16d159d461ab24d52bd054d2105
CN(C)CCOc1cccc2cc[nH]c12.Cc1cccc(OCCN2CCCC2)c1[N+](=O)[O-]>>c1cc(OCCN2CCCC2)c2[nH]ccc2c1
CN(CCOC1=C(C(=CC=C1)C)[N+](=O)[O-])C.CC=1C(=C(OCCN2CCCC2)C=CC1)[N+](=O)[O-].N1C=CC2=CC=CC(=C12)OCCN(C)C>>N1(CCCC1)CCOC=1C=CC=C2C=CNC12
CN(C)CCOc1cccc2c1[nH][cH:14][cH:15]2.C[c:16]1[c:12]([N+:13](=O)[O-])[c:3]([O:4][CH2:5][CH2:6][N:7]2[CH2:8][CH2:9][CH2:10][CH2:11]2)[cH:2][cH:1][cH:17]1>>[cH:1]1[cH:2][c:3]([O:4][CH2:5][CH2:6][N:7]2[CH2:8][CH2:9][CH2:10][CH2:11]2)[c:12]2[nH:13][cH:14][cH:15][c:16]2[cH:17]1
CN(C)CCOc1cccc2cc[nH]c12.Cc1cccc(OCCN2CCCC2)c1[N+](=O)[O-]
c1cc(OCCN2CCCC2)c2[nH]ccc2c1
null
null
null
Functional Group Interconversion
OtherReaction
12424c63d3fa01c4059a4bb31ed39ed8757d1e260dc5a3bac3db3fa104cc1975
8c13929085ad4895d58ee34dc1e3d96ab276ec2f67337a1d5210ac6e1bd98088
c1cc(OCCN2CCCC2)c2[nH]ccc2c1
C-N(-C)-C-C-O-c1:c:c:c:c2:[cH;D2;+0:1]:[cH;D2;+0:2]:[nH]:c:1:2.C-[c;H0;D3;+0:3](:[c:4]:[c:5]):[c:6](-[N+;H0;D3:7](=O)-[O-]):[c:8]>>[c:5]:[c:4]:[c;H0;D3;+0:3]1:[cH;D2;+0:1]:[cH;D2;+0:2]:[nH;D2;+0:7]:[c:6]:1:[c:8]
null
[]
null
null
null
null
The following compound was prepared in a similar fashion, starting with dimethyl-[2-(3-methyl-2-nitro-phenoxy)-ethyl]-amine rather than 1-[2-(3-methyl-2-nitrophenoxy)-ethyl]-pyrrolidine: [2-(1H-indol-7-yloxy)-ethyl]-dimethyl-amine (69%), MS: 205 (M+H)+ Conditions: See reaction.notes.procedure_details. Workup: The follo...
10.6084/m9.figshare.5104873.v1
null
Ether.Nitro group.Tertiary amine
null
c1ccc2[nH]ccc2c1.c1ccccc1
c1ccc2[nH]ccc2c1
C1CC[NH]C1.c1ccc2[nH]ccc2c1
HO-
null
null
null
CN(C)CCOc1cccc2cc[nH]c12.Cc1cccc(OCCN2CCCC2)c1[N+](=O)[O-]>>c1cc(OCCN2CCCC2)c2[nH]ccc2c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-657f79367abc4069a1261c2d77576d05
CI.CN(CCOc1cccc2c(S(=O)(=O)c3ccccc3F)c[nH]c12)C(=O)OC(C)(C)C>>CN(CCOc1cccc2c(S(=O)(=O)c3ccccc3F)cn(C)c12)C(=O)OC(C)(C)C
C(C)(C)(C)OC(N(C)CCOC=1C=CC=C2C(=CNC12)S(=O)(=O)C1=C(C=CC=C1)F)=O.[H-].[Na+].CI>>C(C)(C)(C)OC(N(C)CCOC=1C=CC=C2C(=CN(C12)C)S(=O)(=O)C1=C(C=CC=C1)F)=O
I[CH3:24].[CH3:1][N:2]([CH2:3][CH2:4][O:5][c:6]1[cH:7][cH:8][cH:9][c:10]2[c:11]([S:12](=[O:13])(=[O:14])[c:15]3[cH:16][cH:17][cH:18][cH:19][c:20]3[F:21])[cH:22][nH:23][c:25]12)[C:26](=[O:27])[O:28][C:29]([CH3:30])([CH3:31])[CH3:32]>>[CH3:1][N:2]([CH2:3][CH2:4][O:5][c:6]1[cH:7][cH:8][cH:9][c:10]2[c:11]([S:12](=[O:13])(=...
CI.CN(CCOc1cccc2c(S(=O)(=O)c3ccccc3F)c[nH]c12)C(=O)OC(C)(C)C
CN(CCOc1cccc2c(S(=O)(=O)c3ccccc3F)cn(C)c12)C(=O)OC(C)(C)C
null
null
CN(C=O)C
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
5ce73e9bd608d5491381e563c654ad03f655de6d7aa46423d6263e854c49919a
7a358c636daddc97c1fb4c29f378044d7eac3f01815d9966e599841f642d631a
O=S(=O)(c1ccccc1)c1c[nH]c2ccccc12
I-[CH3;D1;+0:1].[c:2]:[c:3]1:[c:4]:[c:5]:[c:6]:[nH;D2;+0:7]:1>>[CH3;D1;+0:1]-[n;H0;D3;+0:7]1:[c:6]:[c:5]:[c:4]:[c:3]:1:[c:2]
null
[]
null
null
10
MINUTE
A dry 25 mL flask equipped with a magnetic stirrer was charged with {2-[3-(2-fluoro-benzenesulfonyl)-1H-indol-7-yloxy]-ethyl}-methyl-carbamic acid tert-butyl ester (0.116 g., 0.258 mmol) and dimethylformamide (5 mL.) This solution was treated with sodium hydride (0.011 g. of 60% suspension in mineral oil, 0.284 mmol) a...
10.6084/m9.figshare.5104873.v1
null
null
null
c1ccc2[nH]ccc2c1
c1c[nH]c2ccccc12
c1ccccc1.c1c[nH]c2ccccc12
HI
CN(C=O)C
null
0.166667
CI.CN(CCOc1cccc2c(S(=O)(=O)c3ccccc3F)c[nH]c12)C(=O)OC(C)(C)C>CN(C=O)C>CN(CCOc1cccc2c(S(=O)(=O)c3ccccc3F)cn(C)c12)C(=O)OC(C)(C)C
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-0e9e8d5c94114eeeb2ac26b063c4d5b9
CC(C)(C)OC(=O)N1CC(COc2cccc3[nH]ccc23)C1>>CN(CCOc1cccc2[nH]ccc12)C(=O)OC(C)(C)C
C(C)(C)(C)OC(=O)N1CC(C1)CO.C(C)(C)(C)OC(=O)N1CC(C1)COC1=C2C=CNC2=CC=C1>>C(C)(C)(C)OC(N(C)CCOC1=C2C=CNC2=CC=C1)=O
C1[N:2]([C:15](=[O:16])[O:17][C:18]([CH3:19])([CH3:20])[CH3:21])[CH2:1][CH:3]1[CH2:4][O:5][c:6]1[cH:7][cH:8][cH:9][c:10]2[nH:11][cH:12][cH:13][c:14]12>>[CH3:1][N:2]([CH2:3][CH2:4][O:5][c:6]1[cH:7][cH:8][cH:9][c:10]2[nH:11][cH:12][cH:13][c:14]12)[C:15](=[O:16])[O:17][C:18]([CH3:19])([CH3:20])[CH3:21]
CC(C)(C)OC(=O)N1CC(COc2cccc3[nH]ccc23)C1
CN(CCOc1cccc2[nH]ccc12)C(=O)OC(C)(C)C
null
null
null
Miscellaneous
OtherReaction
7e6a6565c453df5d5d90babf757b6ca136771d4877777d8a0e0fb7358084654f
b932663ddba91899c323dafb4072eae107b143d8b23ee72dc5710c79986212ad
c1ccc2[nH]ccc2c1
[#8:1]-[C:2]-[CH;D3;+0:3]1-C-[N;H0;D3;+0:4](-[C:5](=[O;D1;H0:6])-[#8:7]-[C:8](-[C;D1;H3:9])(-[C;D1;H3:10])-[C;D1;H3:11])-[CH2;D2;+0:12]-1>>[#8:1]-[C:2]-[CH2;D2;+0:3]-[N;H0;D3;+0:4](-[CH3;D1;+0:12])-[C:5](=[O;D1;H0:6])-[#8:7]-[C:8](-[C;D1;H3:9])(-[C;D1;H3:10])-[C;D1;H3:11]
null
[]
null
null
null
null
In a similar manner, using 3-hydroxymethyl-azetidine-1-carboxylic acid tert-butyl ester in place of (2-hydroxy-ethyl)-methyl-carbamic acid tert-butyl ester, 3-(1H-Indol-4-yloxymethyl)-azetidine-1-carboxylic acid tert-butyl ester was prepared, (25%), (M−H)−=301. Conditions: See reaction.notes.procedure_details. Workup: ...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester
Carbamic ester
C1C[NH]C1
null
c1ccc2[nH]ccc2c1
Other
null
null
null
CC(C)(C)OC(=O)N1CC(COc2cccc3[nH]ccc23)C1>>CN(CCOc1cccc2[nH]ccc12)C(=O)OC(C)(C)C
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-0598c4a6efe64da582219cf0fd57ed5b
CN(CCOc1cccc2c1cc(S(=O)(=O)c1ccccc1)n2C(=O)OC(C)(C)C)C(=O)OC(C)(C)C>>CNCCOc1cccc2[nH]c(S(=O)(=O)c3ccccc3)cc12
C(C)(C)(C)OC(=O)N1C(=CC2=C(C=CC=C12)OCCN(C)C(=O)OC(C)(C)C)S(=O)(=O)C1=CC=CC=C1.Cl>>Cl.C1(=CC=CC=C1)S(=O)(=O)C=1NC2=CC=CC(=C2C1)OCCNC
CC(C)(C)OC(=O)[N:2]([CH3:1])[CH2:3][CH2:4][O:5][c:6]1[cH:7][cH:8][cH:9][c:10]2[n:11](C(=O)OC(C)(C)C)[c:12]([S:13](=[O:14])(=[O:15])[c:16]3[cH:17][cH:18][cH:19][cH:20][cH:21]3)[cH:22][c:23]12>>[CH3:1][NH:2][CH2:3][CH2:4][O:5][c:6]1[cH:7][cH:8][cH:9][c:10]2[nH:11][c:12]([S:13](=[O:14])(=[O:15])[c:16]3[cH:17][cH:18][cH:19...
CN(CCOc1cccc2c1cc(S(=O)(=O)c1ccccc1)n2C(=O)OC(C)(C)C)C(=O)OC(C)(C)C
CNCCOc1cccc2[nH]c(S(=O)(=O)c3ccccc3)cc12
null
null
CCO
Reduction
OtherReaction
e71913f257fed84ef2af126ddaecf582cb32eea15a3c3c94fef05ab526c72196
b6e7823586033bfbc03f4d0c8dc7543754c419d00fed6ec047b5fd9adf5eea30
O=S(=O)(c1ccccc1)c1cc2ccccc2[nH]1
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1](-[C;D1;H3:2])-[C:3]-[C:4].C-C(-C)(-C)-O-C(=O)-[n;H0;D3;+0:5]1:[c:6](:[c:7]):[c:8]:[c:9]:[c:10]:1-[#16:11]>>[#16:11]-[c:10]1:[c:9]:[c:8]:[c:6](:[c:7]):[nH;D2;+0:5]:1.[C:4]-[C:3]-[NH;D2;+0:1]-[C;D1;H3:2]
null
[]
100
CELSIUS
null
null
2-Benzenesulfonyl-4-[2-(tert-butoxycarbonyl-methyl-amino)-ethoxy]-indole-1-carboxylic acid tert-butyl ester (0.250 g., 0.5 mmol) from Step 3 was dissolved in 5 mL EtOH. To this solution was added 1 mL of 2M ethanolic hydrogen chloride solution. The reaction mixture was heated at 100° C. for 35 minutes. Upon cooling to ...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Ether.Boc.Boc
Secondary amine
c1cc2ccccc2[nH]1
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.c1ccccc1
HO-
CCO
100
null
CN(CCOc1cccc2c1cc(S(=O)(=O)c1ccccc1)n2C(=O)OC(C)(C)C)C(=O)OC(C)(C)C>CCO>CNCCOc1cccc2[nH]c(S(=O)(=O)c3ccccc3)cc12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-97136cb279ec42c48c1676e51c7624a8
CN(CCOc1cccc2cc(S(=O)(=O)c3ccccc3)n(C(=O)OC(C)(C)C)c12)C(=O)OC(C)(C)C>>CNCCOc1cccc2cc(S(=O)(=O)c3ccccc3)[nH]c12
C(C)(C)(C)OC(=O)N1C(=CC2=CC=CC(=C12)OCCN(C)C(=O)OC(C)(C)C)S(=O)(=O)C1=CC=CC=C1.Cl>>Cl.C1(=CC=CC=C1)S(=O)(=O)C=1NC2=C(C=CC=C2C1)OCCNC
CC(C)(C)OC(=O)[N:2]([CH3:1])[CH2:3][CH2:4][O:5][c:6]1[cH:7][cH:8][cH:9][c:10]2[cH:11][c:12]([S:13](=[O:14])(=[O:15])[c:16]3[cH:17][cH:18][cH:19][cH:20][cH:21]3)[n:22](C(=O)OC(C)(C)C)[c:23]12>>[CH3:1][NH:2][CH2:3][CH2:4][O:5][c:6]1[cH:7][cH:8][cH:9][c:10]2[cH:11][c:12]([S:13](=[O:14])(=[O:15])[c:16]3[cH:17][cH:18][cH:19...
CN(CCOc1cccc2cc(S(=O)(=O)c3ccccc3)n(C(=O)OC(C)(C)C)c12)C(=O)OC(C)(C)C
CNCCOc1cccc2cc(S(=O)(=O)c3ccccc3)[nH]c12
null
null
CCO
Reduction
OtherReaction
e71913f257fed84ef2af126ddaecf582cb32eea15a3c3c94fef05ab526c72196
b6e7823586033bfbc03f4d0c8dc7543754c419d00fed6ec047b5fd9adf5eea30
O=S(=O)(c1ccccc1)c1cc2ccccc2[nH]1
C-C(-C)(-C)-O-C(=O)-[N;H0;D3;+0:1](-[C;D1;H3:2])-[C:3]-[C:4].C-C(-C)(-C)-O-C(=O)-[n;H0;D3;+0:5]1:[c:6](-[#16:7]):[c:8]:[c:9]:[c:10]:1:[c:11]>>[#16:7]-[c:6]1:[c:8]:[c:9]:[c:10](:[c:11]):[nH;D2;+0:5]:1.[C:4]-[C:3]-[NH;D2;+0:1]-[C;D1;H3:2]
null
[]
100
CELSIUS
null
null
2-Benzenesulfonyl-7-[2-(tert-butoxycarbonyl-methyl-amino)-ethoxy]-indole-1-carboxylic acid tert-butyl ester (0.230 g., 0.43 mmol) from the above step was dissolved in 5 mL EtOH. To this solution was added 1 mL of 2M ethanolic hydrogen chloride solution. The reaction mixture was heated at 100° C. for 35 minutes. Upon co...
10.6084/m9.figshare.5104873.v1
null
Carbamic ester.Ether.Ether.Boc.Boc
Secondary amine
c1cc2ccccc2[nH]1
c1ccc2[nH]ccc2c1
c1ccc2[nH]ccc2c1.c1ccccc1
HO-
CCO
100
null
CN(CCOc1cccc2cc(S(=O)(=O)c3ccccc3)n(C(=O)OC(C)(C)C)c12)C(=O)OC(C)(C)C>CCO>CNCCOc1cccc2cc(S(=O)(=O)c3ccccc3)[nH]c12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-586c518b04a74c998bdaf509414209bb
N#CCBr.Oc1cccc2cc[nH]c12>>N#CCOc1cccc2cc[nH]c12
BrCC#N.OC=1C=CC=C2C=CNC12.C([O-])([O-])=O.[K+].[K+]>>N1C=CC2=CC=CC(=C12)OCC#N
Br[CH2:3][C:2]#[N:1].[OH:4][c:5]1[cH:6][cH:7][cH:8][c:9]2[cH:10][cH:11][nH:12][c:13]12>>[N:1]#[C:2][CH2:3][O:4][c:5]1[cH:6][cH:7][cH:8][c:9]2[cH:10][cH:11][nH:12][c:13]12
N#CCBr.Oc1cccc2cc[nH]c12
N#CCOc1cccc2cc[nH]c12
null
null
C(C)#N
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
7e1040116e3a4cf0e8ec5cc7865388d9cd0efabce6d320a1c25a36e411018d8b
d5f4610d46ccc0478471c5bc0fb862644eaf764bbc5d93badb39d54f6ec8e0a5
c1ccc2[nH]ccc2c1
Br-[CH2;D2;+0:1]-[C:2]#[N;D1;H0:3].[OH;D1;+0:4]-[c:5](:[c:6]):[c:7](:[c:8]):[#7;a:9]:[c:10]>>[N;D1;H0:3]#[C:2]-[CH2;D2;+0:1]-[O;H0;D2;+0:4]-[c:5](:[c:6]):[c:7](:[c:8]):[#7;a:9]:[c:10]
null
[]
0
CELSIUS
3
HOUR
In a 100 mL roundbottom flask equipped with a magnetic stirrer and rubber septum, 7-hydroxy-1H-indole (1.66 g., 12.48 mmol) was dissolved 50 mL anhydrous acetonitrile. The flask was charged with potassium carbonate (6.88 g., 49.9 mmol) and cooled to 0° C. While stirring, bromoacetonitrile (1.64 g., 13.73 mmol) was adde...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Aromatic alcohol
Ether
null
null
c1ccc2[nH]ccc2c1
HBr
C(C)#N
0
3
N#CCBr.Oc1cccc2cc[nH]c12>C(C)#N>N#CCOc1cccc2cc[nH]c12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-28ef4f87f29444f4ab29c44206c85e6f
NCCOc1cccc2c(S(=O)(=O)c3ccccc3F)c[nH]c12>>NCCOc1cccc2c(S(=O)(=O)c3ccccc3F)c[nH]c12
O.O.O.O.O.O.O.O.O.O.S(=O)(=O)([O-])[O-].[Na+].[Na+].FC1=C(C=CC=C1)S(=O)(=O)C1=CNC2=C(C=CC=C12)OCCN.Cl>>Cl.FC1=C(C=CC=C1)S(=O)(=O)C1=CNC2=C(C=CC=C12)OCCN
[NH2:2][CH2:3][CH2:4][O:5][c:6]1[cH:7][cH:8][cH:9][c:10]2[c:11]([S:12](=[O:13])(=[O:14])[c:15]3[cH:16][cH:17][cH:18][cH:19][c:20]3[F:21])[cH:22][nH:23][c:24]12>>[NH2:2][CH2:3][CH2:4][O:5][c:6]1[cH:7][cH:8][cH:9][c:10]2[c:11]([S:12](=[O:13])(=[O:14])[c:15]3[cH:16][cH:17][cH:18][cH:19][c:20]3[F:21])[cH:22][nH:23][c:24]12
NCCOc1cccc2c(S(=O)(=O)c3ccccc3F)c[nH]c12
NCCOc1cccc2c(S(=O)(=O)c3ccccc3F)c[nH]c12
null
null
C(C)O
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
O=S(=O)(c1ccccc1)c1c[nH]c2ccccc12
null
11
[{"value": 11.0, "product": "Cl.FC1=C(C=CC=C1)S(=O)(=O)C1=CNC2=C(C=CC=C12)OCCN", "details": "PERCENTYIELD", "is_desired": false}]
0
CELSIUS
1
HOUR
A dry 25 mL roundbottom flask was equipped with a magnetic stirrer and purged with argon gas. To this was added via syringe a solution of [3-(2-fluoro-benzenesulfonyl)-1H-indol-7-yloxy]-acetonitrile in 10 mL of anhydrous THF. The flask was cooled to 0° C. and lithium aluminum hydride solution was added (1 mL of 1M solu...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
c1ccccc1.c1ccc2[nH]ccc2c1
null
C(C)O
0
1
NCCOc1cccc2c(S(=O)(=O)c3ccccc3F)c[nH]c12>C(C)O>NCCOc1cccc2c(S(=O)(=O)c3ccccc3F)c[nH]c12
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-c726936bb48143acb2070697d2b01b54
NS(=O)(=O)c1ccc(Br)s1>>N#Cc1ccc(S(N)(=O)=O)s1
CO.CN(C=O)C.O.C(C)(=O)OCC.BrC1=CC=C(S1)S(=O)(=O)N.CN(C=O)C>>C(#N)C1=CC=C(S1)S(=O)(=O)N
Br[c:3]1[cH:4][cH:5][c:6]([S:7]([NH2:8])(=[O:9])=[O:10])[s:11]1>>[N:1]#[C:2][c:3]1[cH:4][cH:5][c:6]([S:7]([NH2:8])(=[O:9])=[O:10])[s:11]1
NS(=O)(=O)c1ccc(Br)s1
N#Cc1ccc(S(N)(=O)=O)s1
null
[C-]#N.[Zn+2].[C-]#N.C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
C(Cl)Cl
Miscellaneous
OtherReaction
ebc2e53b7bb2dea43338a6ebf76eca4e26da1c045bb86707697af7150e28603d
73a96fe5e833259ca394a42f82d6cc2ee7231bcde92d95030d2893b90c3fef76
c1ccsc1
Br-[c;H0;D3;+0:1]1:[#16;a:2]:[c:3]:[c:4]:[c:5]:1>>[N;D1;H0:6]#[C:7]-[c;H0;D3;+0:1]1:[#16;a:2]:[c:3]:[c:4]:[c:5]:1
null
[]
null
null
15
MINUTE
A mixture of 5-bromothiophene-2-sulfonamide (0.50 g, 2.1 mmol), zinc cyanide (0.25 g, 2.1 mmol), tetrakis(triphenylphosphine)palladium(0) (0.072 g, 0.06 mmol) in dimethylformamide (5 mL, anhydrous) is placed under microwave radiation (under nitrogen atmosphere, 160° C.) for 15 min. Thin layer chromatography (5% methyl ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
Nitrile
c1ccsc1
c1ccsc1
c1ccsc1
Br-
[C-]#N.[Zn+2].[C-]#N.C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C(Cl)Cl
null
0.25
NS(=O)(=O)c1ccc(Br)s1>[C-]#N.[Zn+2].[C-]#N.C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.C(Cl)Cl>N#Cc1ccc(S(N)(=O)=O)s1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-7b3ef08a6ec846058fe20b3dbccc2c1d
NS(=O)(=O)c1ccc(Br)s1.[C]=O>>COC(=O)c1ccc(S(N)(=O)=O)s1
[C]=O.BrC1=CC=C(S1)S(=O)(=O)N.C(C)N(CC)CC.C1(=CC=CC=C1)P(CCCP(C1=CC=CC=C1)C1=CC=CC=C1)C1=CC=CC=C1.C(C)(=O)OCC>>COC(=O)C1=CC=C(S1)S(=O)(=O)N
Br[c:5]1[cH:6][cH:7][c:8]([S:9]([NH2:10])(=[O:11])=[O:12])[s:13]1.[C:3]=[O:4]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([S:9]([NH2:10])(=[O:11])=[O:12])[s:13]1
NS(=O)(=O)c1ccc(Br)s1.[C]=O
COC(=O)c1ccc(S(N)(=O)=O)s1
null
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-]
CO.CN(C=O)C.[Cl-].[Na+].O
Acylation
OtherReaction
4a22c433c553169ad2d2a5923b627757ce76160edc71987c02daeeccd0e27f17
843b64a5a526f70107d024a7003b94aa750190d2759e9e4e7ac8f05f2eb068bc
c1ccsc1
Br-[c;H0;D3;+0:1]1:[#16;a:2]:[c:3]:[c:4]:[c:5]:1.[C;H0;D1;+0:6]=[O;D1;H0:7]>>[C;D1;H3:8]-[#8:9]-[C;H0;D3;+0:6](=[O;D1;H0:7])-[c;H0;D3;+0:1]1:[#16;a:2]:[c:3]:[c:4]:[c:5]:1
null
[]
100
CELSIUS
8
HOUR
A mixture of 5-bromothiophene-2-sulfonamide (0.50 g, 2.1 mmol), triethyl amine (1 mL), methanol (1 mL), palladium acetate (0.046 g, 2.1 mmol) and 1,3-bis(diphenylphosphino) propane (0.085 g, 2.1 mmol) (addition in that order) in dimethylformamide (5 mL, anhydrous) is saturated with carbon monoxide gas, at room temperat...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
Ester
c1ccsc1
c1ccsc1
c1ccsc1
Br-
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].CO.CN(C=O)C.[Cl-].[Na+].O
100
8
NS(=O)(=O)c1ccc(Br)s1.[C]=O>C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-].CO.CN(C=O)C.[Cl-].[Na+].O>COC(=O)c1ccc(S(N)(=O)=O)s1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-ee96dca7353343b0ab451e1a1c0600f7
NS(=O)(=O)c1cc(Cl)c(Br)s1>>NS(=O)(=O)c1cc(Cl)cs1
BrC1=C(C=C(S1)S(=O)(=O)N)Cl>>ClC=1C=C(SC1)S(=O)(=O)N
Br[c:9]1[c:7]([Cl:8])[cH:6][c:5]([S:2]([NH2:1])(=[O:3])=[O:4])[s:10]1>>[NH2:1][S:2](=[O:3])(=[O:4])[c:5]1[cH:6][c:7]([Cl:8])[cH:9][s:10]1
NS(=O)(=O)c1cc(Cl)c(Br)s1
NS(=O)(=O)c1cc(Cl)cs1
null
[Zn]
CC(=O)O
Functional Group Interconversion
Aromatic dehalogenation
305afd15d586f55c801d6d4acac09c00bdce7795c11721d329be09a54571e3e8
56de34d4a44cb25d9380269ee5e138b0f24b40a3a0db22c5508049dc775a861f
c1ccsc1
Br-[c;H0;D3;+0:1]1:[#16;a:2]:[c:3]:[c:4]:[c:5]:1-[Cl;D1;H0:6]>>[Cl;D1;H0:6]-[c:5]1:[c:4]:[c:3]:[#16;a:2]:[cH;D2;+0:1]:1
52
[{"value": 52.0, "product": "ClC=1C=C(SC1)S(=O)(=O)N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 51.2, "product": "ClC=1C=C(SC1)S(=O)(=O)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
120
CELSIUS
6
HOUR
To a stirred solution of 5-bromo-4-chlorothiophene-2-sulfonamide (2.4 g, 8.7 mmol) in AcOH (20 mL) is added zinc dust (1.7 g, 26.0 mmol). The reaction mixture is heated to 120° C. for 6 hr. After 6 hr, the mixture is filtered and neutralized with 1 M NaOH. The aqueous layer is extracted with EtOAc (2×100 mL). The combi...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1ccsc1
c1ccsc1
c1ccsc1
Br-
[Zn].CC(=O)O
120
6
NS(=O)(=O)c1cc(Cl)c(Br)s1>[Zn].CC(=O)O>NS(=O)(=O)c1cc(Cl)cs1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-d567173a966040fe8fce61a1b01b4a96
Cc1cc(S(N)(=O)=O)sc1Br>>Cc1csc(S(N)(=O)=O)c1
BrC1=C(C=C(S1)S(=O)(=O)N)C>>CC=1C=C(SC1)S(=O)(=O)N
Br[c:3]1[c:2]([CH3:1])[cH:10][c:5]([S:6]([NH2:7])(=[O:8])=[O:9])[s:4]1>>[CH3:1][c:2]1[cH:3][s:4][c:5]([S:6]([NH2:7])(=[O:8])=[O:9])[cH:10]1
Cc1cc(S(N)(=O)=O)sc1Br
Cc1csc(S(N)(=O)=O)c1
null
[Zn]
CC(=O)O
Functional Group Interconversion
Aromatic dehalogenation
305afd15d586f55c801d6d4acac09c00bdce7795c11721d329be09a54571e3e8
56de34d4a44cb25d9380269ee5e138b0f24b40a3a0db22c5508049dc775a861f
c1ccsc1
Br-[c;H0;D3;+0:1]1:[#16;a:2]:[c:3]:[c:4]:[c:5]:1-[C;D1;H3:6]>>[C;D1;H3:6]-[c:5]1:[c:4]:[c:3]:[#16;a:2]:[cH;D2;+0:1]:1
43
[{"value": 43.0, "product": "CC=1C=C(SC1)S(=O)(=O)N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 42.0, "product": "CC=1C=C(SC1)S(=O)(=O)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
To a stirred solution of 5-bromo-4-methylthiophene-2-sulfonamide (3.1 g, 12.1 mmol) in AcOH (30 mL) is added zinc dust (2.4 g, 36.2 mmol). The reaction mixture is heated to reflux for 8 hr. After 8 hr, the reaction mixture is cooled and filtered. The filtrate is neutralized with 1 M NaOH. The aqueous layer is extracted...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide
null
c1ccsc1
c1ccsc1
c1ccsc1
Br-
[Zn].CC(=O)O
null
8
Cc1cc(S(N)(=O)=O)sc1Br>[Zn].CC(=O)O>Cc1csc(S(N)(=O)=O)c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-565e2ecce6004964ad51bb958a449fdc
COc1ccsc1.C[Si](C)(C)Cl>>COc1ccsc1[Si](C)(C)C
[Li]CCCC.COC1=CSC=C1.Cl[Si](C)(C)C>>C[Si](C=1SC=CC1OC)(C)C
[CH3:1][O:2][c:3]1[cH:4][cH:5][s:6][cH:7]1.Cl[Si:8]([CH3:9])([CH3:10])[CH3:11]>>[CH3:1][O:2][c:3]1[cH:4][cH:5][s:6][c:7]1[Si:8]([CH3:9])([CH3:10])[CH3:11]
COc1ccsc1.C[Si](C)(C)Cl
COc1ccsc1[Si](C)(C)C
null
null
CCOCC
Functional Group Interconversion
OtherReaction
9d3a5d1aca09168804224649157f4cdeee866ecdd1eb4932b5bd9bc687e334ae
62b25486659a0c3b8981491307676661488416039e4a601c8996c7216be92cf1
c1ccsc1
Cl-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[C;D1;H3:4].[#8:5]-[c:6]1:[c:7]:[c:8]:[#16;a:9]:[cH;D2;+0:10]:1>>[#8:5]-[c:6]1:[c:7]:[c:8]:[#16;a:9]:[c;H0;D3;+0:10]:1-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[C;D1;H3:4]
82
[{"value": 82.0, "product": "C[Si](C=1SC=CC1OC)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 81.6, "product": "C[Si](C=1SC=CC1OC)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-70
CELSIUS
2
HOUR
A solution of n-BuLi (19.7 mL of 1.6 M in hexanes, 31.5 mmol) is added dropwise to a solution of 3-methoxythiophene (3.0 g, 26.3 mmol) in anhydrous Et2O (20 mL) under nitrogen at −70° C. The mixture is stirred at −70° C. for 2 hr. Chlorotrimethylsilane (4.5 mL, 35.4 mmol) is added slowly to the solution. The mixture is...
10.6084/m9.figshare.5104873.v1
null
Silyl protective group
Silyl protective group
c1ccsc1
c1ccsc1
c1ccsc1
HCl
CCOCC
-70
2
COc1ccsc1.C[Si](C)(C)Cl>CCOCC>COc1ccsc1[Si](C)(C)C
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-4011bed5f5294dad8742b47fef93d11e
COc1cc(S(N)(=O)=O)sc1[Si](C)(C)C>>COc1csc(S(N)(=O)=O)c1
C[Si](C1=C(C=C(S1)S(=O)(=O)N)OC)(C)C.[F-].C(CCC)[N+](CCCC)(CCCC)CCCC>>COC=1C=C(SC1)S(=O)(=O)N
C[Si](C)(C)[c:4]1[c:3]([O:2][CH3:1])[cH:11][c:6]([S:7]([NH2:8])(=[O:9])=[O:10])[s:5]1>>[CH3:1][O:2][c:3]1[cH:4][s:5][c:6]([S:7]([NH2:8])(=[O:9])=[O:10])[cH:11]1
COc1cc(S(N)(=O)=O)sc1[Si](C)(C)C
COc1csc(S(N)(=O)=O)c1
null
null
C1CCOC1
Miscellaneous
OtherReaction
fb103db3c69bbb9797704a2b619962ad5a7046c2eac756eb173e3698fc27e14b
dc52a720480da1d65217db7d5178c684d09e72e99cbbe1f9f67cca818c9ff2e9
c1ccsc1
C-[Si](-C)(-C)-[c;H0;D3;+0:1]1:[#16;a:2]:[c:3]:[c:4]:[c:5]:1-[#8:6]>>[#8:6]-[c:5]1:[c:4]:[c:3]:[#16;a:2]:[cH;D2;+0:1]:1
86
[{"value": 86.0, "product": "COC=1C=C(SC1)S(=O)(=O)N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 85.7, "product": "COC=1C=C(SC1)S(=O)(=O)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
To a solution of 5-trimethylsilyl-4-methoxythiophene-2-sulfonamide (770 mg, 2.90 mmol) in THF (10 mL) is added a solution of tetra-butylammonium fluoride (17.4 mL of 1 M in THF, 17.4 mmol). The reaction mixture is stirred at room temperature for 2 hr. The THF is removed under reduced pressure. The residue is dissolved ...
10.6084/m9.figshare.5104873.v1
null
Silyl protective group
null
c1ccsc1
c1ccsc1
c1ccsc1
Other
C1CCOC1
null
2
COc1cc(S(N)(=O)=O)sc1[Si](C)(C)C>C1CCOC1>COc1csc(S(N)(=O)=O)c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-691061cfa6dd4a19863f6daf18e6a0b4
COc1csc(S(N)(=O)=O)c1.O=C1CCC(=O)N1Br>>COc1cc(S(N)(=O)=O)sc1Br
COC=1C=C(SC1)S(=O)(=O)N.BrN1C(CCC1=O)=O>>BrC1=C(C=C(S1)S(=O)(=O)N)OC
[CH3:1][O:2][c:3]1[cH:4][c:5]([S:6]([NH2:7])(=[O:8])=[O:9])[s:10][cH:11]1.O=C1CCC(=O)N1[Br:12]>>[CH3:1][O:2][c:3]1[cH:4][c:5]([S:6]([NH2:7])(=[O:8])=[O:9])[s:10][c:11]1[Br:12]
COc1csc(S(N)(=O)=O)c1.O=C1CCC(=O)N1Br
COc1cc(S(N)(=O)=O)sc1Br
null
null
C(Cl)Cl
Functional Group Interconversion
Bromination
a42d5393618d10b862dd7bd471fa3f4459c31017c8714cafb4e591f8ed4a8052
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
c1ccsc1
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#8:2]-[c:3]1:[c:4]:[c:5]:[#16;a:6]:[cH;D2;+0:7]:1>>[#8:2]-[c:3]1:[c:4]:[c:5]:[#16;a:6]:[c;H0;D3;+0:7]:1-[Br;H0;D1;+0:1]
82.1
[{"value": 82.0, "product": "BrC1=C(C=C(S1)S(=O)(=O)N)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 82.1, "product": "BrC1=C(C=C(S1)S(=O)(=O)N)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
7
HOUR
To a solution of 4-methoxythiophene-2-sulfonamide (240 mg, 1.24 mmol) in CH2Cl2 (40 mL) is added N-bromosuccinimide (287 mg, 1.61 mmol). The reaction mixture is stirred at 0° C. for 7 hr. After 7 hr, the reaction mixture is diluted with CH2Cl2 (150 mL). The organic layer is washed with brine then dried (Na2SO4), filter...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1ccsc1.C1CCNC1
c1ccsc1
c1ccsc1
HO-
C(Cl)Cl
0
7
COc1csc(S(N)(=O)=O)c1.O=C1CCC(=O)N1Br>C(Cl)Cl>COc1cc(S(N)(=O)=O)sc1Br
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-9191d766b42f4cd196abeaea614de401
CSc1ccsc1.C[Si](C)(C)Cl>>CSc1ccsc1[Si](C)(C)C
[Li]CCCC.CSC1=CSC=C1.Cl[Si](C)(C)C>>C[Si](C=1SC=CC1SC)(C)C
[CH3:1][S:2][c:3]1[cH:4][cH:5][s:6][cH:7]1.Cl[Si:8]([CH3:9])([CH3:10])[CH3:11]>>[CH3:1][S:2][c:3]1[cH:4][cH:5][s:6][c:7]1[Si:8]([CH3:9])([CH3:10])[CH3:11]
CSc1ccsc1.C[Si](C)(C)Cl
CSc1ccsc1[Si](C)(C)C
null
null
CCOCC
Functional Group Interconversion
OtherReaction
9d3a5d1aca09168804224649157f4cdeee866ecdd1eb4932b5bd9bc687e334ae
62b25486659a0c3b8981491307676661488416039e4a601c8996c7216be92cf1
c1ccsc1
Cl-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[C;D1;H3:4].[#16:5]-[c:6]1:[c:7]:[c:8]:[#16;a:9]:[cH;D2;+0:10]:1>>[#16:5]-[c:6]1:[c:7]:[c:8]:[#16;a:9]:[c;H0;D3;+0:10]:1-[Si;H0;D4;+0:1](-[C;D1;H3:2])(-[C;D1;H3:3])-[C;D1;H3:4]
48
[{"value": 48.0, "product": "C[Si](C=1SC=CC1SC)(C)C", "details": "PERCENTYIELD", "is_desired": false}]
-70
CELSIUS
2
HOUR
A solution of n-BuLi (5.3 mL of 1.6 M in hexanes, 8.5 mmol) is added dropwise to a solution of 3-methylsulfanylthiophene (1.0 g, 7.7 mmol) in anhydrous Et2O (8 mL) under nitrogen at −70° C. The mixture is stirred at −70° C. for 2 hr. Chlorotrimethylsilane (1.5 mL) is added slowly to the reaction mixture. The mixture is...
10.6084/m9.figshare.5104873.v1
null
Silyl protective group
Silyl protective group
c1ccsc1
c1ccsc1
c1ccsc1
HCl
CCOCC
-70
2
CSc1ccsc1.C[Si](C)(C)Cl>CCOCC>CSc1ccsc1[Si](C)(C)C
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-a67ac309ad074910a843d2a272c82903
CSc1cc(S(N)(=O)=O)sc1[Si](C)(C)C>>CSc1csc(S(N)(=O)=O)c1
C[Si](C1=C(C=C(S1)S(=O)(=O)N)SC)(C)C.[F-].C(CCC)[N+](CCCC)(CCCC)CCCC>>CSC=1C=C(SC1)S(=O)(=O)N
C[Si](C)(C)[c:4]1[c:3]([S:2][CH3:1])[cH:11][c:6]([S:7]([NH2:8])(=[O:9])=[O:10])[s:5]1>>[CH3:1][S:2][c:3]1[cH:4][s:5][c:6]([S:7]([NH2:8])(=[O:9])=[O:10])[cH:11]1
CSc1cc(S(N)(=O)=O)sc1[Si](C)(C)C
CSc1csc(S(N)(=O)=O)c1
null
null
C1CCOC1
Miscellaneous
OtherReaction
fb103db3c69bbb9797704a2b619962ad5a7046c2eac756eb173e3698fc27e14b
dc52a720480da1d65217db7d5178c684d09e72e99cbbe1f9f67cca818c9ff2e9
c1ccsc1
C-[Si](-C)(-C)-[c;H0;D3;+0:1]1:[#16;a:2]:[c:3]:[c:4]:[c:5]:1-[#16:6]>>[#16:6]-[c:5]1:[c:4]:[c:3]:[#16;a:2]:[cH;D2;+0:1]:1
82
[{"value": 82.0, "product": "CSC=1C=C(SC1)S(=O)(=O)N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 81.7, "product": "CSC=1C=C(SC1)S(=O)(=O)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3
HOUR
To a solution of 5-trimethylsilyl-4-methylsulfanylthiophene-2-sulfonamide (660 mg, 2.34 mmol) in THF (10 mL) is added a solution of tetra-butylammonium fluoride (14.0 mL of 1 M in THF, 14.0 mmol). The reaction mixture is stirred at room temperature for 3 hr. The THF is removed under reduced pressure and the residue is ...
10.6084/m9.figshare.5104873.v1
null
Silyl protective group
null
c1ccsc1
c1ccsc1
c1ccsc1
Other
C1CCOC1
null
3
CSc1cc(S(N)(=O)=O)sc1[Si](C)(C)C>C1CCOC1>CSc1csc(S(N)(=O)=O)c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-0942076c4c394968b6a28abbf66cf3d6
CSc1csc(S(N)(=O)=O)c1.O=C1CCC(=O)N1Br>>CSc1cc(S(N)(=O)=O)sc1Br
CSC=1C=C(SC1)S(=O)(=O)N.BrN1C(CCC1=O)=O.[OH-].[Na+]>>BrC1=C(C=C(S1)S(=O)(=O)N)SC
[CH3:1][S:2][c:3]1[cH:4][c:5]([S:6]([NH2:7])(=[O:8])=[O:9])[s:10][cH:11]1.O=C1CCC(=O)N1[Br:12]>>[CH3:1][S:2][c:3]1[cH:4][c:5]([S:6]([NH2:7])(=[O:8])=[O:9])[s:10][c:11]1[Br:12]
CSc1csc(S(N)(=O)=O)c1.O=C1CCC(=O)N1Br
CSc1cc(S(N)(=O)=O)sc1Br
null
null
C(Cl)(Cl)Cl.CC(=O)O
Functional Group Interconversion
Bromination
a42d5393618d10b862dd7bd471fa3f4459c31017c8714cafb4e591f8ed4a8052
0e444576b73669992a4073cc3f7b10ed52cb9df09f9f8e4042e39e6a602aa390
c1ccsc1
O=C1-C-C-C(=O)-N-1-[Br;H0;D1;+0:1].[#16:2]-[c:3]1:[c:4]:[c:5]:[#16;a:6]:[cH;D2;+0:7]:1>>[#16:2]-[c:3]1:[c:4]:[c:5]:[#16;a:6]:[c;H0;D3;+0:7]:1-[Br;H0;D1;+0:1]
70
[{"value": 70.0, "product": "BrC1=C(C=C(S1)S(=O)(=O)N)SC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 69.4, "product": "BrC1=C(C=C(S1)S(=O)(=O)N)SC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
7
HOUR
To a solution of 4-methylsulfanylthiophene-2-sulfonamide (210 mg, 1.00 mmol) in CHCl3 (10 mL) and AcOH (10 mL) is added N-bromosuccinimide (231 mg, 1.30 mmol). The reaction mixture is stirred at room temperature for 7 hr. After 7 hr, the reaction mixture is neutralized with 1 M NaOH and the solution is extracted with E...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide.Tertiary amide
Aromatic halide
c1ccsc1.C1CCNC1
c1ccsc1
c1ccsc1
HO-
C(Cl)(Cl)Cl.CC(=O)O
null
7
CSc1csc(S(N)(=O)=O)c1.O=C1CCC(=O)N1Br>C(Cl)(Cl)Cl.CC(=O)O>CSc1cc(S(N)(=O)=O)sc1Br
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-55e97c7bfb3c4a3b8e73d36580db020d
Nc1ccc(Br)cc1Br>>N#Cc1ccc(Br)cc1Br
Cl.BrC1=C(N)C=CC(=C1)Br.[Cu](C#N)C#N.C(C)(C)(C)ON=O>>BrC1=C(C#N)C=CC(=C1)Br
N[c:3]1[cH:4][cH:5][c:6]([Br:7])[cH:8][c:9]1[Br:10]>>[N:1]#[C:2][c:3]1[cH:4][cH:5][c:6]([Br:7])[cH:8][c:9]1[Br:10]
Nc1ccc(Br)cc1Br
N#Cc1ccc(Br)cc1Br
null
null
CS(=O)C
Miscellaneous
OtherReaction
803ab123dd5297cb23d9a6340952837f436e629c02fa01486d208bb7e2b4e208
fb780e6912aa057969f5ca1e3a4b096c038904d81ac37783ac8b177057c79824
c1ccccc1
N-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[Br;D1;H0:5]):[c:6]>>[Br;D1;H0:5]-[c:4](:[c:6]):[c;H0;D3;+0:1](-[C:7]#[N;D1;H0:8]):[c:2]:[c:3]
31
[{"value": 31.0, "product": "BrC1=C(C#N)C=CC(=C1)Br", "details": "PERCENTYIELD", "is_desired": false}, {"value": 31.0, "product": "BrC1=C(C#N)C=CC(=C1)Br", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
45
CELSIUS
1
HOUR
Copper cyanide (2.32 g, 25.9 mmol) is added to stirred anhydrous dimethylsulfoxide (50 mL) at 60° C. to form a clear solution, followed by the addition of tert-butylnitrite (7.1 mL, 59.7 mmol) all at once. A solution of 2,4-dibromoaniline 21 (5.0 g, 19.9 mmol) in anhydrous dimethylsulfoxide (30 mL) is added dropwise, v...
10.6084/m9.figshare.5104873.v1
null
Primary amine
Nitrile
c1ccccc1
c1ccccc1
c1ccccc1
null
CS(=O)C
45
1
Nc1ccc(Br)cc1Br>CS(=O)C>N#Cc1ccc(Br)cc1Br
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-09dbf5b4d43440c18a10b96ec12ac8d1
Br.Nc1cc(Cl)ccc1C(=O)O>>O=C(O)c1ccc(Cl)cc1Br
NC1=C(C(=O)O)C=CC(=C1)Cl.Br.[N+](=O)([O-])[O-].[Na+]>>BrC1=C(C(=O)O)C=CC(=C1)Cl
[BrH:11].N[c:10]1[c:4]([C:2](=[O:1])[OH:3])[cH:5][cH:6][c:7]([Cl:8])[cH:9]1>>[O:1]=[C:2]([OH:3])[c:4]1[cH:5][cH:6][c:7]([Cl:8])[cH:9][c:10]1[Br:11]
Br.Nc1cc(Cl)ccc1C(=O)O
O=C(O)c1ccc(Cl)cc1Br
null
[Cu](Br)Br
O
Miscellaneous
OtherReaction
976fb3f0996203ccf639edc3dd63ebf792dabe502fe07eb66206f5ee630d746b
1129c10513c603d2647e51dd9713063aaf10bd8a364ed275b9b93c32624e3ba4
c1ccccc1
N-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[C:5](=[O;D1;H0:6])-[O;D1;H1:7]):[c:8].[BrH;D0;+0:9]>>[Br;H0;D1;+0:9]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[C:5](=[O;D1;H0:6])-[O;D1;H1:7]):[c:8]
59
[{"value": 59.0, "product": "BrC1=C(C(=O)O)C=CC(=C1)Cl", "details": "PERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
An aqueous solution of sodium nitrate (2.21 g) in water (15 mL) is added dropwise to a stirred, ice-cooled mixture of 2-amino-4-chlorobenzoic acid (5.00 g, 29.1 mmol) and 48% hydrobromic acid (150 mL) in water (150 mL). The resultant mixture is stirred for 2 hr at 0° C. Then it is treated dropwise with an aqueous solut...
10.6084/m9.figshare.5104873.v1
null
Primary amine
Aromatic halide
c1ccccc1
c1ccccc1
c1ccccc1
Other
[Cu](Br)Br.O
null
8
Br.Nc1cc(Cl)ccc1C(=O)O>[Cu](Br)Br.O>O=C(O)c1ccc(Cl)cc1Br
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-aee51196cc95496697f04b34ba5c4da1
CN(C)C=O.CO.Cc1ccc(Br)c(Cl)c1>>COC(=O)c1ccc(C)cc1Cl
BrC1=C(C=C(C=C1)C)Cl.C1(=CC=CC=C1)P(CCCP(C1=CC=CC=C1)C1=CC=CC=C1)C1=CC=CC=C1.C(C)N(CC)CC.CO.CN(C=O)C>>ClC1=C(C(=O)OC)C=CC(=C1)C
CN(C)[CH:3]=[O:4].[CH3:1][OH:2].Br[c:5]1[cH:6][cH:7][c:8]([CH3:9])[cH:10][c:11]1[Cl:12]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([CH3:9])[cH:10][c:11]1[Cl:12]
CN(C)C=O.CO.Cc1ccc(Br)c(Cl)c1
COC(=O)c1ccc(C)cc1Cl
null
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-]
null
Acylation
OtherReaction
ba60403ad7d45c466fc5a7cbbd7ecd8e4611ae8790a58d10f5ebcfca5f732591
3e4a6d9d1b66fe5eba87f87fea1406f49c9bbd0c9181018bc2624480752f7ca5
c1ccccc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[Cl;D1;H0:5]):[c:6].C-N(-C)-[CH;D2;+0:7]=[O;D1;H0:8].[C;D1;H3:9]-[OH;D1;+0:10]>>[C;D1;H3:9]-[O;H0;D2;+0:10]-[C;H0;D3;+0:7](=[O;D1;H0:8])-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[Cl;D1;H0:5]):[c:6]
28
[{"value": 28.0, "product": "ClC1=C(C(=O)OC)C=CC(=C1)C", "details": "PERCENTYIELD", "is_desired": false}]
80
CELSIUS
null
null
To 4-bromo-3-chlorotoluene (4.97 g, 24.2 mmol) in dimethylformamide (25 mL) is added palladium acetate (0.54 g, 2.42 mmol), 1,3-bis(diphenylphosphino)propane (0.998 g, 2.42 mmol), triethylamine (12.5 mL) and methanol (12.5 mL). The reaction vessel is evacuated and purged three times with carbon monoxide gas. A balloon ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Tertiary amide.Methanol
Ester
c1ccccc1
c1ccccc1
c1ccccc1
HBr
C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-]
80
null
CN(C)C=O.CO.Cc1ccc(Br)c(Cl)c1>C(C)(=O)[O-].[Pd+2].C(C)(=O)[O-]>COC(=O)c1ccc(C)cc1Cl
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-cea61636641643349db50d2479857ff0
COC(=O)c1ccc(C)cc1Cl>>Cc1ccc(C(=O)O)c(Cl)c1
ClC1=C(C(=O)OC)C=CC(=C1)C.[OH-].[Li+]>>ClC1=C(C(=O)O)C=CC(=C1)C
C[O:8][C:6]([c:5]1[cH:4][cH:3][c:2]([CH3:1])[cH:11][c:9]1[Cl:10])=[O:7]>>[CH3:1][c:2]1[cH:3][cH:4][c:5]([C:6](=[O:7])[OH:8])[c:9]([Cl:10])[cH:11]1
COC(=O)c1ccc(C)cc1Cl
Cc1ccc(C(=O)O)c(Cl)c1
null
null
O.O1CCCC1
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccccc1
C-[O;H0;D2;+0:1]-[C:2](=[O;D1;H0:3])-[c:4]>>[O;D1;H0:3]=[C:2](-[OH;D1;+0:1])-[c:4]
100
[{"value": 100.0, "product": "ClC1=C(C(=O)O)C=CC(=C1)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 99.7, "product": "ClC1=C(C(=O)O)C=CC(=C1)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
50
CELSIUS
null
null
To methyl 2-chloro-4-methylbenzoate (1.00 g, 5.42 mmol) in tetrahydrofuran (10 mL) methyl alcohol (5 mL) and water (2.5 mL) is added 2N lithium hydroxide (8.12 mL, 16.2 mmol). The reaction mixture is heated at 50° C. for 2.5 hr, cooled to room temperature, and then quenched with 5N hydrochloric acid (3.24 mL). The mixt...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1
Other
O.O1CCCC1
50
null
COC(=O)c1ccc(C)cc1Cl>O.O1CCCC1>Cc1ccc(C(=O)O)c(Cl)c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-d146ffc4743f46cfb9a96289a70a2846
CCOC(=O)CC(=O)C(F)(F)F.COS(=O)(=O)c1ccc(C)cc1>>CCOC(=O)C=C(OC)C(F)(F)F
C1(=CC=C(C=C1)S(=O)(=O)OC)C.FC(C(CC(=O)OCC)=O)(F)F.C([O-])([O-])=O.[Cs+].[Cs+]>>C(C)OC(C=C(C(F)(F)F)OC)=O
[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH2:6][C:7](=[O:8])[C:10]([F:11])([F:12])[F:13].Cc1ccc(S(=O)(=O)O[CH3:9])cc1>>[CH3:1][CH2:2][O:3][C:4](=[O:5])[CH:6]=[C:7]([O:8][CH3:9])[C:10]([F:11])([F:12])[F:13]
CCOC(=O)CC(=O)C(F)(F)F.COS(=O)(=O)c1ccc(C)cc1
CCOC(=O)C=C(OC)C(F)(F)F
null
null
O.CN(C)C=O
Heteroatom Alkylation and Arylation
OtherReaction
0dc58f4d3ac1f54d21a41413dfb3bbdac23e0786bbf3d7a4617d6b94a0282309
fa98111d5b9696af827e0889b49ab9e37ed100109e38ecbec1b7162fb7d02238
null
C-c1:c:c:c(-S(=O)(=O)-O-[CH3;D1;+0:1]):c:c:1.[C:2]-[#8:3]-[C:4](=[O;D1;H0:5])-[CH2;D2;+0:6]-[C;H0;D3;+0:7](=[O;H0;D1;+0:8])-[C:9](-[F;D1;H0:10])(-[F;D1;H0:11])-[F;D1;H0:12]>>[C:2]-[#8:3]-[C:4](=[O;D1;H0:5])-[CH;D2;+0:6]=[C;H0;D3;+0:7](-[O;H0;D2;+0:8]-[CH3;D1;+0:1])-[C:9](-[F;D1;H0:10])(-[F;D1;H0:11])-[F;D1;H0:12]
56
[{"value": 56.0, "product": "C(C)OC(C=C(C(F)(F)F)OC)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 55.4, "product": "C(C)OC(C=C(C(F)(F)F)OC)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
70
CELSIUS
1
HOUR
To a solution of ethyl 4,4,4-trifluoroacetoacetate (12 mL, 82 mmol) in DMF (80 mL) is added cesium carbonate (26.4 g, 82 mmol). The reaction mixture is heated to 70° C. A solution of methyl p-toluenesulfonate (13.5 mL, 90 mmol) in DMF (30 mL) is then added dropwise during 30 min and the reaction mixture is stirred for ...
10.6084/m9.figshare.5104873.v1
null
Tosylate.Ketone.Ester
Ester.Ether
c1ccccc1
null
null
TsOH.HO-
O.CN(C)C=O
70
1
CCOC(=O)CC(=O)C(F)(F)F.COS(=O)(=O)c1ccc(C)cc1>O.CN(C)C=O>CCOC(=O)C=C(OC)C(F)(F)F
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-3615251532314f45bc7131ceaf9195cd
CCOC(=O)C=C(OC)C(F)(F)F.COC(=O)CS>>COC(=O)c1sc(C(F)(F)F)cc1O
C(C)OC(C=C(C(F)(F)F)OC)=O.C(CS)(=O)OC.OS(=O)(=O)O.[OH-].[K+]>>COC(=O)C=1SC(=CC1O)C(F)(F)F
CCO[C:13]([CH:12]=[C:7](OC)[C:8]([F:9])([F:10])[F:11])=[O:14].[CH3:1][O:2][C:3](=[O:4])[CH2:5][SH:6]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[s:6][c:7]([C:8]([F:9])([F:10])[F:11])[cH:12][c:13]1[OH:14]
CCOC(=O)C=C(OC)C(F)(F)F.COC(=O)CS
COC(=O)c1sc(C(F)(F)F)cc1O
null
null
CO.O
Aromatic Heterocycle Formation
OtherReaction
77dd272d651c2798c3c9424a71f8bba3dd13045a7eea6e89b42541b338cbddd5
cb4d41d978c3d8970a717baa1898aebe45e360b2a07c34662ddbc01c205b9792
c1ccsc1
C-C-O-[C;H0;D3;+0:1](=[O;H0;D1;+0:2])-[CH;D2;+0:3]=[C;H0;D3;+0:4](-O-C)-[C:5](-[F;D1;H0:6])(-[F;D1;H0:7])-[F;D1;H0:8].[C;D1;H3:9]-[#8:10]-[C:11](=[O;D1;H0:12])-[CH2;D2;+0:13]-[SH;D1;+0:14]>>[C;D1;H3:9]-[#8:10]-[C:11](=[O;D1;H0:12])-[c;H0;D3;+0:13]1:[s;H0;D2;+0:14]:[c;H0;D3;+0:4](-[C:5](-[F;D1;H0:6])(-[F;D1;H0:7])-[F;D1...
91.2
[{"value": 91.0, "product": "COC(=O)C=1SC(=CC1O)C(F)(F)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 91.2, "product": "COC(=O)C=1SC(=CC1O)C(F)(F)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
A solution of 4,4,4-trifluoro-3-methoxy-but-2-enoic acid ethyl ester (9.6 g, 48.5 mmol) and methyl thioglycolate (4.3 mL, 48.5 mmol) in MeOH (75 mL) is cooled to 5° C. A solution of KOH (3.3 g, 58.2 mmol) in MeOH (75 mL) is then added over 30 min. The reaction mixture is stirred overnight at room temperature. The react...
10.6084/m9.figshare.5104873.v1
null
Ester.Ester.Ether.Aliphatic thiol
Ester.Aromatic alcohol
null
c1ccsc1
c1ccsc1
HO-
CO.O
null
8
CCOC(=O)C=C(OC)C(F)(F)F.COC(=O)CS>CO.O>COC(=O)c1sc(C(F)(F)F)cc1O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-97bd380cae1c4e708eb824535de2f9eb
Clc1nnnn1-c1ccccc1.Oc1csc(C(F)(F)F)c1>>FC(F)(F)c1cc(Oc2nnnn2-c2ccccc2)cs1
FC(C1=CC(=CS1)O)(F)F.ClC1=NN=NN1C1=CC=CC=C1.C(=O)([O-])[O-].[K+].[K+]>>C1(=CC=CC=C1)N1N=NN=C1OC1=CSC(=C1)C(F)(F)F
Cl[c:9]1[n:10][n:11][n:12][n:13]1-[c:14]1[cH:15][cH:16][cH:17][cH:18][cH:19]1.[F:1][C:2]([F:3])([F:4])[c:5]1[cH:6][c:7]([OH:8])[cH:20][s:21]1>>[F:1][C:2]([F:3])([F:4])[c:5]1[cH:6][c:7]([O:8][c:9]2[n:10][n:11][n:12][n:13]2-[c:14]2[cH:15][cH:16][cH:17][cH:18][cH:19]2)[cH:20][s:21]1
Clc1nnnn1-c1ccccc1.Oc1csc(C(F)(F)F)c1
FC(F)(F)c1cc(Oc2nnnn2-c2ccccc2)cs1
null
null
CC(=O)C
Heteroatom Alkylation and Arylation
Williamson Ether Synthesis
b0b5fa75f8d32dfc2c1c81f67556be0cd9accee81c6065b457dea599b9ba080f
27e9a6bab4e3ed54aeb6be4d84cb1c0170208288795e252a46e57e44ecc064f0
c1ccc(-n2nnnc2Oc2ccsc2)cc1
Cl-[c;H0;D3;+0:1]1:[#7;a:2]:[#7;a:3]:[#7;a:4]:[#7;a:5]:1-[c:6].[OH;D1;+0:7]-[c:8]1:[c:9]:[#16;a:10]:[c:11]:[c:12]:1>>[c:6]-[#7;a:5]1:[#7;a:4]:[#7;a:3]:[#7;a:2]:[c;H0;D3;+0:1]:1-[O;H0;D2;+0:7]-[c:8]1:[c:9]:[#16;a:10]:[c:11]:[c:12]:1
68
[{"value": 68.0, "product": "C1(=CC=CC=C1)N1N=NN=C1OC1=CSC(=C1)C(F)(F)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 67.3, "product": "C1(=CC=CC=C1)N1N=NN=C1OC1=CSC(=C1)C(F)(F)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 5-trifluoromethyl-thiophen-3-ol (2.0 g, 11.9 mmol) in dry acetone (480 mL) containing 5-chloro-1-phenyl-1H-tetrazole (2.1 g, 11.9 mmol) and K2CO3 (3.3 g, 23.8 mmol) is maintained at reflux with careful exclusion of moisture overnight. The acetone is removed under reduced pressure and the residue is partit...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Aromatic alcohol
Ether
c1nnn[nH]1
c1nnn[nH]1
c1ccsc1.c1nnn[nH]1.c1ccccc1
HCl
CC(=O)C
null
null
Clc1nnnn1-c1ccccc1.Oc1csc(C(F)(F)F)c1>CC(=O)C>FC(F)(F)c1cc(Oc2nnnn2-c2ccccc2)cs1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-83b360ca114c47f9936ef07085d51598
NS(=O)(=O)c1ccc(-n2nnnc2Oc2cc(C(F)(F)F)sc2S(N)(=O)=O)cc1>>NS(=O)(=O)c1ccc(C(F)(F)F)s1
S(N)(=O)(=O)C1=CC=C(C=C1)N1N=NN=C1OC1=C(SC(=C1)C(F)(F)F)S(=O)(=O)N.O.CCO.C(=O)O>>FC(C1=CC=C(S1)S(=O)(=O)N)(F)F
NS(=O)(=O)c1ccc(-n2nnnc2O[c:6]2[c:5]([S:2]([NH2:1])(=[O:3])=[O:4])[s:13][c:8]([C:9]([F:10])([F:11])[F:12])[cH:7]2)cc1>>[NH2:1][S:2](=[O:3])(=[O:4])[c:5]1[cH:6][cH:7][c:8]([C:9]([F:10])([F:11])[F:12])[s:13]1
NS(=O)(=O)c1ccc(-n2nnnc2Oc2cc(C(F)(F)F)sc2S(N)(=O)=O)cc1
NS(=O)(=O)c1ccc(C(F)(F)F)s1
null
[Pd]
C1=CC=CC=C1
Reduction
OtherReaction
ba5bfc5b3482059af1846468354831d20c4ccc44b6a82b8e0c59a2e82917dd0f
aa7cf63c080af8644a576d884d07cafb9f1b7f6e4bb39c7f680496e99a92bb91
c1ccsc1
N-S(=O)(=O)-c1:c:c:c(-n2:n:n:n:c:2-O-[c;H0;D3;+0:1]2:[c:2]:[c:3](-[C:4](-[F;D1;H0:5])(-[F;D1;H0:6])-[F;D1;H0:7]):[#16;a:8]:[c:9]:2-[#16:10]):c:c:1>>[#16:10]-[c:9]1:[#16;a:8]:[c:3](-[C:4](-[F;D1;H0:5])(-[F;D1;H0:6])-[F;D1;H0:7]):[c:2]:[cH;D2;+0:1]:1
17
[{"value": 17.0, "product": "FC(C1=CC=C(S1)S(=O)(=O)N)(F)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 16.6, "product": "FC(C1=CC=C(S1)S(=O)(=O)N)(F)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
80
CELSIUS
null
null
To a solution of 3-[1-(4-sulfamoyl-phenyl)-1H-tetrazol-5-yloxy]-5-trifluoromethyl-thiophene-2-sulfonamide (210 mg, 0.47 mmol) in benzene (50 mL) is added H2O (2 mL), EtOH (3 mL), formic acid (2 mL) and 10% palladium on carbon (350 mg). The mixture is heated to 80° C. overnight. The reaction mixture is cooled to room te...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Ether
null
c1ccccc1.c1nnn[nH]1.c1ccsc1
c1ccsc1
c1ccsc1
HO-
[Pd].C1=CC=CC=C1
80
null
NS(=O)(=O)c1ccc(-n2nnnc2Oc2cc(C(F)(F)F)sc2S(N)(=O)=O)cc1>[Pd].C1=CC=CC=C1>NS(=O)(=O)c1ccc(C(F)(F)F)s1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-084376ff6cbd402bbcddd99c0de3c3d7
NS(=O)(=O)c1ccc(Br)s1.O=C(O)c1ccc(Br)cc1Cl>>O=C(NS(=O)(=O)c1ccc(Br)s1)c1ccc(Br)cc1Cl
CC=1C=CC(=CC1)S(=O)(=O)O.BrC1=CC=C(S1)S(=O)(=O)N.BrC1=CC(=C(C(=O)O)C=C1)Cl>>BrC1=CC(=C(C(=O)NS(=O)(=O)C=2SC(=CC2)Br)C=C1)Cl
[NH2:3][S:4](=[O:5])(=[O:6])[c:7]1[cH:8][cH:9][c:10]([Br:11])[s:12]1.O[C:2](=[O:1])[c:13]1[cH:14][cH:15][c:16]([Br:17])[cH:18][c:19]1[Cl:20]>>[O:1]=[C:2]([NH:3][S:4](=[O:5])(=[O:6])[c:7]1[cH:8][cH:9][c:10]([Br:11])[s:12]1)[c:13]1[cH:14][cH:15][c:16]([Br:17])[cH:18][c:19]1[Cl:20]
NS(=O)(=O)c1ccc(Br)s1.O=C(O)c1ccc(Br)cc1Cl
O=C(NS(=O)(=O)c1ccc(Br)s1)c1ccc(Br)cc1Cl
null
null
ClCCl
Acylation
Carboxylic acid with primary amine to amide
195a412a8235704efe2985cdc18467ba661e632bab7b61944399ecc813e32a09
5e4665bad9c6f58dddd98c5f95e436c640b4c0118b04efea5cd58c7d1755401d
O=C(NS(=O)(=O)c1cccs1)c1ccccc1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5].[#16;a:6]:[c:7]-[#16:8](-[NH2;D1;+0:9])(=[O;D1;H0:10])=[O;D1;H0:11]>>[#16;a:6]:[c:7]-[#16:8](=[O;D1;H0:10])(=[O;D1;H0:11])-[NH;D2;+0:9]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[c:3](:[c:4]):[c:5]
null
[]
null
null
72
HOUR
An 8 mL reaction vial is charged with 4-bromo-2-chlorobenzoic acid (0.39 mmol, 1.5 eq) and 2.0 mL of dichloromethane. A stock solution (4.0 mL) containing 5-bromothiophene-2-sulfonamide (0.26 mmol, 1 eq) and N,N-[dimethyl]-4-aminopyridine (48 mg, 0.39 mmol, 1.5 eq) in dichloromethane is added, followed by 0.261 g carbo...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Carboxylic acid
Sulfonamide.Secondary amide
null
null
c1ccsc1.c1ccccc1
HO-
ClCCl
null
72
NS(=O)(=O)c1ccc(Br)s1.O=C(O)c1ccc(Br)cc1Cl>ClCCl>O=C(NS(=O)(=O)c1ccc(Br)s1)c1ccc(Br)cc1Cl
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-9cde62dad74542a8b096bc1839d1215f
COCCOCCOCCO.O=C(Cl)C1CC1>>COCCOCCOCCOC(=O)C1CC1
COCCOCCOCCO.C(C)N(CC)CC.C1(CC1)C(=O)Cl>>C1(CC1)C(=O)OCCOCCOCCOC
[CH3:1][O:2][CH2:3][CH2:4][O:5][CH2:6][CH2:7][O:8][CH2:9][CH2:10][OH:11].Cl[C:12](=[O:13])[CH:14]1[CH2:15][CH2:16]1>>[CH3:1][O:2][CH2:3][CH2:4][O:5][CH2:6][CH2:7][O:8][CH2:9][CH2:10][O:11][C:12](=[O:13])[CH:14]1[CH2:15][CH2:16]1
COCCOCCOCCO.O=C(Cl)C1CC1
COCCOCCOCCOC(=O)C1CC1
null
null
ClCCl
Acylation
Schotten-Baumann to ester
6cefe709828c5bd4655f254e75d5dff9e8876e192e7dd47256c1bc0067bc5291
d8a7643b81ed07a6f633aa99465180dfa0565e61ae25aef36338ebb9837c9cef
C1CC1
Cl-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]1-[C:4]-[C:5]-1.[C:6]-[C:7]-[OH;D1;+0:8]>>[C:6]-[C:7]-[O;H0;D2;+0:8]-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3]1-[C:4]-[C:5]-1
null
[]
0
CELSIUS
1
HOUR
Triethylene glycol monomethyl ether (1.1 eq, 5.26 mmol, 0.84 ml), triethylamine (1.1 eq, 5.26 mmol, 0.73 ml) was taken in a 10 ml round bottom flask and dichloromethane (3 ml) was added. This mixture was cooled to 0° C. and then cyclopropanecarbonyl chloride (4.78 mmol, 0.5 g, 0.43 ml) was added in a dropwise fashion m...
10.6084/m9.figshare.5104873.v1
null
Acyl halide.Primary alcohol
Ester
null
null
C1CC1
HCl
ClCCl
0
1
COCCOCCOCCO.O=C(Cl)C1CC1>ClCCl>COCCOCCOCCOC(=O)C1CC1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-cdfc09446c49400d80ac411e2e633a6a
CCN(CC)CC.CS(=O)(=O)Cl.OCCc1ccc(O)cc1>>CS(=O)(=O)OCCc1ccc(OS(C)(=O)=O)cc1
C(C)N(CC)CC.OC1=CC=C(C=C1)CCO.CS(=O)(=O)Cl>>CS(=O)(=O)OCCC1=CC=C(C=C1)OS(=O)(=O)C
CCN(CC)C[CH3:14].Cl[S:2]([CH3:1])(=[O:3])=[O:4].[OH:5][CH2:6][CH2:7][c:8]1[cH:9][cH:10][c:11]([OH:12])[cH:17][cH:18]1>>[CH3:1][S:2](=[O:3])(=[O:4])[O:5][CH2:6][CH2:7][c:8]1[cH:9][cH:10][c:11]([O:12][S:13]([CH3:14])(=[O:15])=[O:16])[cH:17][cH:18]1
CCN(CC)CC.CS(=O)(=O)Cl.OCCc1ccc(O)cc1
CS(=O)(=O)OCCc1ccc(OS(C)(=O)=O)cc1
null
null
C(Cl)Cl
Oxidation
OtherReaction
c36003d3b803e6ac0bbdc324c0694f01c1c5ae153a9aa61e12ae47160d56be56
adf4599ac843f34885822a3073d4ca4e8ae92d6092b8cb127254061af10f08be
c1ccccc1
C-C-N(-C-C)-C-[CH3;D1;+0:1].Cl-[S;H0;D4;+0:2](-[C;D1;H3:3])(=[O;D1;H0:4])=[O;D1;H0:5].[C:6]-[C:7]-[OH;D1;+0:8].[OH;D1;+0:9]-[c:10](:[c:11]):[c:12]>>[CH3;D1;+0:1]-[#16:13](=[O;D1;H0:14])(=[O;D1;H0:15])-[O;H0;D2;+0:9]-[c:10](:[c:11]):[c:12].[C:6]-[C:7]-[O;H0;D2;+0:8]-[S;H0;D4;+0:2](-[C;D1;H3:3])(=[O;D1;H0:4])=[O;D1;H0:5]
null
[]
-20
CELSIUS
null
null
2-(4-Hydroxyphenyl)ethanol(356 g, 2.58 mol, 1.0 eq) was dissolved in methylene chloride (3500 ml) and triethyl amine (653 g, 6.44 mol, 2.5 eq). The mixture was cooled to −20° C. Methanesulfonyl chloride (657 g, 5.74 mol. 2.2 eq) was then added keeping the temperature between −25° C. and −15° C. When the conversion was ...
10.6084/m9.figshare.5104873.v1
null
Primary alcohol.Aromatic alcohol.Tertiary amine.Sulfonyl halide
Mesylate.Mesylate
null
null
c1ccccc1
HCl
C(Cl)Cl
-20
null
CCN(CC)CC.CS(=O)(=O)Cl.OCCc1ccc(O)cc1>C(Cl)Cl>CS(=O)(=O)OCCc1ccc(OS(C)(=O)=O)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-cc6cc8363cff42a4af4528dcc64a7236
CCOC(=O)[C@H](Cc1ccc(OCCc2ccc(OS(C)(=O)=O)cc2)cc1)OCC>>CCO[C@@H](Cc1ccc(OCCc2ccc(OS(C)(=O)=O)cc2)cc1)C(=O)O
[OH-].[Li+].C(C)O[C@H](C(=O)OCC)CC1=CC=C(C=C1)OCCC1=CC=C(C=C1)OS(=O)(=O)C.O1CCCC1.O>>C(C)O[C@H](C(=O)O)CC1=CC=C(C=C1)OCCC1=CC=C(C=C1)OS(=O)(=O)C
CC[O:28][C:26]([C@@H:4]([O:3][CH2:2][CH3:1])[CH2:5][c:6]1[cH:7][cH:8][c:9]([O:10][CH2:11][CH2:12][c:13]2[cH:14][cH:15][c:16]([O:17][S:18]([CH3:19])(=[O:20])=[O:21])[cH:22][cH:23]2)[cH:24][cH:25]1)=[O:27]>>[CH3:1][CH2:2][O:3][C@@H:4]([CH2:5][c:6]1[cH:7][cH:8][c:9]([O:10][CH2:11][CH2:12][c:13]2[cH:14][cH:15][c:16]([O:17]...
CCOC(=O)[C@H](Cc1ccc(OCCc2ccc(OS(C)(=O)=O)cc2)cc1)OCC
CCO[C@@H](Cc1ccc(OCCc2ccc(OS(C)(=O)=O)cc2)cc1)C(=O)O
null
null
C(C)(=O)OCC
Deprotection
Ester saponification (alkyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
c1ccc(CCOc2ccccc2)cc1
C-C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
null
[]
null
null
30
MINUTE
To the oil of ethyl (S)-2-ethoxy-3-[4-[[4-(methylsulfonyloxy)phenethyl]oxy]phenyl]propanoate (723 g(71.2% assay), 1.18 mol, 1.0 eq) was added tetrahydrofuran (THF) (3900 ml). When a homogenous solution was formed, water (900 ml) was added. The mixture was cooled to +10° C. Lithium hydroxide solution (390 ml, 4 M, 1.45 ...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
c1ccccc1.c1ccccc1
Other
C(C)(=O)OCC
null
0.5
CCOC(=O)[C@H](Cc1ccc(OCCc2ccc(OS(C)(=O)=O)cc2)cc1)OCC>C(C)(=O)OCC>CCO[C@@H](Cc1ccc(OCCc2ccc(OS(C)(=O)=O)cc2)cc1)C(=O)O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-fbb70cf1aa6d4f91b0623384d82a6ec4
BrBr.O=C1Cc2ccccc2N1>>O=C1Cc2cc(Br)ccc2N1
O.N1C(CC2=CC=CC=C12)=O.C(C)(=O)[O-].[Na+].BrBr>>BrC=1C=C2CC(NC2=CC1)=O
Br[Br:7].[O:1]=[C:2]1[CH2:3][c:4]2[cH:5][cH:6][cH:8][cH:9][c:10]2[NH:11]1>>[O:1]=[C:2]1[CH2:3][c:4]2[cH:5][c:6]([Br:7])[cH:8][cH:9][c:10]2[NH:11]1
BrBr.O=C1Cc2ccccc2N1
O=C1Cc2cc(Br)ccc2N1
null
null
CCOC(=O)C.C(Cl)(Cl)Cl
Functional Group Interconversion
Bromination
e5aad40fc3ec640bed45a7119ff569558b20c39979304f365dafdbc5ae4e4cd4
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
O=C1Cc2ccccc2N1
Br-[Br;H0;D1;+0:1].[c:2]:[c:3]:[cH;D2;+0:4]:[c:5]:[c:6]>>[Br;H0;D1;+0:1]-[c;H0;D3;+0:4](:[c:3]:[c:2]):[c:5]:[c:6]
97.3
[{"value": 96.0, "product": "BrC=1C=C2CC(NC2=CC1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 97.3, "product": "BrC=1C=C2CC(NC2=CC1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
A solution of oxindole (2.0 g, 15.0 mmol) and sodium acetate (2.1 g, 25.5 mmol) in CHCl3 (20 cm3) was treated with bromine (2.4 g, 15.0 mmol) in CHCl3 (10 cm3). After 30 min. the mixture was allowed to warm to RT and stirred for 1 h. The reaction mixture was diluted with EtOAc (500 cm3) and poured into water. The aqueo...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2c(c1)CCN2
c1ccc2c(c1)CCN2
c1ccc2c(c1)CCN2
HBr
CCOC(=O)C.C(Cl)(Cl)Cl
null
0.5
BrBr.O=C1Cc2ccccc2N1>CCOC(=O)C.C(Cl)(Cl)Cl>O=C1Cc2cc(Br)ccc2N1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-73b578707101440ab23e494441247e5a
O=C1Cc2cc(Br)ccc2N1.O=[N+]([O-])c1cccc(B(O)O)c1>>O=C1Cc2cc(-c3cccc([N+](=O)[O-])c3)ccc2N1
BrC=1C=C2CC(NC2=CC1)=O.[N+](=O)([O-])C=1C=C(C=CC1)B(O)O.C([O-])([O-])=O.[K+].[K+]>>[N+](=O)([O-])C=1C=C(C=CC1)C=1C=C2CC(NC2=CC1)=O
Br[c:6]1[cH:5][c:4]2[c:18]([cH:17][cH:16]1)[NH:19][C:2](=[O:1])[CH2:3]2.OB(O)[c:7]1[cH:8][cH:9][cH:10][c:11]([N+:12](=[O:13])[O-:14])[cH:15]1>>[O:1]=[C:2]1[CH2:3][c:4]2[cH:5][c:6](-[c:7]3[cH:8][cH:9][cH:10][c:11]([N+:12](=[O:13])[O-:14])[cH:15]3)[cH:16][cH:17][c:18]2[NH:19]1
O=C1Cc2cc(Br)ccc2N1.O=[N+]([O-])c1cccc(B(O)O)c1
O=C1Cc2cc(-c3cccc([N+](=O)[O-])c3)ccc2N1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.COCCOC
C-C Coupling
Suzuki coupling with boronic acids
9791290dea007c134587598bd16674eb122eb7281e427c61b6d8f55d72a5f584
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Cc2cc(-c3ccccc3)ccc2N1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:8]:[c:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9]:[c:10]
65
[{"value": 65.0, "product": "[N+](=O)([O-])C=1C=C(C=CC1)C=1C=C2CC(NC2=CC1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 6.5, "product": "[N+](=O)([O-])C=1C=C(C=CC1)C=1C=C2CC(NC2=CC1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
5-bromo-2-indolinone (1.08 g, 5.09 mmol) and tetrakistriphenyl phosphine Pd (0) (0.273 g) were stirred under an atmosphere of nitrogen in ethylene glycol dimethyl ether (35 mL). After 15 minutes, 3-nitrophenyl boronic acid (1.70 g, 10.2 mmol) was added, followed by potassium carbonate (4.24 g, 30.7 mmol) in water (15 m...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2c(c1)CCN2.c1ccccc1
c1ccc2c(c1)CCN2.c1ccccc1
c1ccc2c(c1)CCN2.c1ccccc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC
null
0.25
O=C1Cc2cc(Br)ccc2N1.O=[N+]([O-])c1cccc(B(O)O)c1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC>O=C1Cc2cc(-c3cccc([N+](=O)[O-])c3)ccc2N1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-30b90ddcbdb4472aae87c4606838feb4
BrBr.CC1C(=O)Nc2ccccc21>>CC1=c2cc(Br)ccc2=NC1=O
C([O-])([O-])=O.[Na+].[Na+].BrBr.CC1C(NC2=CC=CC=C12)=O.C(C)(=O)[O-].[Na+]>>BrC1=CC2=C(C(N=C2C=C1)=O)C
Br[Br:6].[CH3:1][CH:2]1[c:3]2[cH:4][cH:5][cH:7][cH:8][c:9]2[NH:10][C:11]1=[O:12]>>[CH3:1][C:2]1=[c:3]2[cH:4][c:5]([Br:6])[cH:7][cH:8][c:9]2=[N:10][C:11]1=[O:12]
BrBr.CC1C(=O)Nc2ccccc21
CC1=c2cc(Br)ccc2=NC1=O
null
null
C(C)(=O)O
Functional Group Interconversion
OtherReaction
f77276f67562534d698ae9969b38604bf6d0631d673dbcf49471739b8fb2dc9c
10d5e9f7ea4e0a6d7c64f3eede8b2722c836d0e851a0ab7fb8f5aa5d2bdff633
O=C1C=c2ccccc2=N1
Br-[Br;H0;D1;+0:1].[C;D1;H3:2]-[CH;D3;+0:3]1-[C:4](=[O;D1;H0:5])-[NH;D2;+0:6]-[c;H0;D3;+0:7]2:[c:8]:[c:9]:[cH;D2;+0:10]:[c:11]:[c;H0;D3;+0:12]:2-1>>[Br;H0;D1;+0:1]-[c;H0;D3;+0:10]1:[c:11]:[c;H0;D3;+0:12]2:[c;H0;D3;+0:7](:[c:8]:[c:9]:1)=[N;H0;D2;+0:6]-[C:4](=[O;D1;H0:5])-[C;H0;D3;+0:3]=2-[C;D1;H3:2]
93.7
[{"value": 93.0, "product": "BrC1=CC2=C(C(N=C2C=C1)=O)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 93.7, "product": "BrC1=CC2=C(C(N=C2C=C1)=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
3.5
HOUR
Under an atmosphere of nitrogen, bromine (0.96 g, 6.0 mmol) in acetic acid (5 cm3) was added drop wise to a solution of 3-methyl-2-indolinone (0.8749 g, 6.0 mmol) (Kende, et al, Synth. Commun., 12, 1, 1982) and sodium acetate (0.50 g, 6.0 mmol) in acetic acid (10 cm3). The reaction was stirred at room temperature for 3...
10.6084/m9.figshare.5104873.v1
null
Secondary amide
Aromatic halide
c1ccc2c(c1)CCN2
C1=c2ccccc2=NC1
C1=c2ccccc2=NC1
HBr
C(C)(=O)O
null
3.5
BrBr.CC1C(=O)Nc2ccccc21>C(C)(=O)O>CC1=c2cc(Br)ccc2=NC1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-f1ad471805684fc5b6ebc2d669085dc4
CC1C(=O)Nc2ccc(Br)cc21>>CC1=c2cc(Br)ccc2=NC1=O
[Cl-].[NH4+].BrC=1C=C2C(C(NC2=CC1)=O)C.[N+](=O)([O-])C=1C=C(C=CC1)B(O)O.C([O-])([O-])=O.[K+].[K+]>>BrC1=CC2=C(C(N=C2C=C1)=O)C
[CH3:1][CH:2]1[c:3]2[cH:4][c:5]([Br:6])[cH:7][cH:8][c:9]2[NH:10][C:11]1=[O:12]>>[CH3:1][C:2]1=[c:3]2[cH:4][c:5]([Br:6])[cH:7][cH:8][c:9]2=[N:10][C:11]1=[O:12]
CC1C(=O)Nc2ccc(Br)cc21
CC1=c2cc(Br)ccc2=NC1=O
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.C(OC)COC
Oxidation
OtherReaction
5888764ac5705b4fccbaa0f333db96bf6faba4a5ea8e8011bddc2ecf15e91da3
951ba0a3ea11fb59b51e8c5a89ac77de7d3f3bdc1496c8df7b8fa4f398d1bd93
O=C1C=c2ccccc2=N1
[C;D1;H3:1]-[CH;D3;+0:2]1-[C:3](=[O;D1;H0:4])-[NH;D2;+0:5]-[c;H0;D3;+0:6]2:[c:7]:[c:8]:[c:9]:[c:10]:[c;H0;D3;+0:11]:2-1>>[C;D1;H3:1]-[C;H0;D3;+0:2]1=[c;H0;D3;+0:11]2:[c:10]:[c:9]:[c:8]:[c:7]:[c;H0;D3;+0:6]:2=[N;H0;D2;+0:5]-[C:3]-1=[O;D1;H0:4]
60.3
[{"value": 47.0, "product": "BrC1=CC2=C(C(N=C2C=C1)=O)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 60.3, "product": "BrC1=CC2=C(C(N=C2C=C1)=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
5-Bromo-3-methyl-1,3-dihydro-indol-2-one (0.50 g, 2.22 mmol) and tetrakis(triphenylphosphine)palladium(0) (0.15 g) were stirred under an atmosphere of nitrogen in dimethoxyethane (18 cm3). After 15 min., 3-nitrophenyl boronic acid (0.74 g, 4.45 mmol) was added, followed by potassium carbonate (1.86 g, 13.5 mmol) in wat...
10.6084/m9.figshare.5104873.v1
null
Secondary amide
null
c1ccc2c(c1)CCN2
C1=c2ccccc2=NC1
C1=c2ccccc2=NC1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.C(OC)COC
null
0.25
CC1C(=O)Nc2ccc(Br)cc21>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.C(OC)COC>CC1=c2cc(Br)ccc2=NC1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-78f0cb74792a4655a3abe774e955057c
CC1(C)C(=O)Nc2ccc(Br)cc21.OB(O)c1cccc(Cl)c1>>CC1(C)C(=O)Nc2ccc(-c3cccc(Cl)c3)cc21
BrC=1C=C2C(C(NC2=CC1)=O)(C)C.ClC=1C=C(C=CC1)B(O)O.C([O-])([O-])=O.[K+].[K+]>>ClC=1C=C(C=CC1)C=1C=C2C(C(NC2=CC1)=O)(C)C
Br[c:10]1[cH:9][cH:8][c:7]2[c:19]([cH:18]1)[C:2]([CH3:1])([CH3:3])[C:4](=[O:5])[NH:6]2.OB(O)[c:11]1[cH:12][cH:13][cH:14][c:15]([Cl:16])[cH:17]1>>[CH3:1][C:2]1([CH3:3])[C:4](=[O:5])[NH:6][c:7]2[cH:8][cH:9][c:10](-[c:11]3[cH:12][cH:13][cH:14][c:15]([Cl:16])[cH:17]3)[cH:18][c:19]21
CC1(C)C(=O)Nc2ccc(Br)cc21.OB(O)c1cccc(Cl)c1
CC1(C)C(=O)Nc2ccc(-c3cccc(Cl)c3)cc21
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.C(OC)COC.[Cl-].[NH4+]
C-C Coupling
Suzuki coupling with boronic acids
9791290dea007c134587598bd16674eb122eb7281e427c61b6d8f55d72a5f584
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Cc2cc(-c3ccccc3)ccc2N1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:8]:[c:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9]:[c:10]
25
[{"value": 25.0, "product": "ClC=1C=C(C=CC1)C=1C=C2C(C(NC2=CC1)=O)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 0.0, "product": "ClC=1C=C(C=CC1)C=1C=C2C(C(NC2=CC1)=O)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
5-bromo-1,3-dihydro-3,3-dimethyl-2H-indol-2-one (0.98 g, 4.07 mol) and, tetrakis(triphenylphosphine)palladium(0) (0.239 g) were stirred under an atmosphere of nitrogen in dimethoxyethane (35 cm3). After 15 min., 3-chlorophenylboronic acid (1.27 g, 8.13 mol) was added, followed by potassium carbonate (3.40 g, 45 mmol) i...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2c(c1)CCN2.c1ccccc1
c1ccc2c(c1)CCN2.c1ccccc1
c1ccc2c(c1)CCN2.c1ccccc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.C(OC)COC.[Cl-].[NH4+]
null
0.25
CC1(C)C(=O)Nc2ccc(Br)cc21.OB(O)c1cccc(Cl)c1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.C(OC)COC.[Cl-].[NH4+]>CC1(C)C(=O)Nc2ccc(-c3cccc(Cl)c3)cc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-31d1fe9f37be4dd1a460278d3b248409
CC1(C)C(=O)Nc2ccc(Br)cc21.O=[N+]([O-])c1cccc(B(O)O)c1>>CC1(C)C(=O)Nc2ccc(-c3cccc([N+](=O)[O-])c3)cc21
[Cl-].[NH4+].BrC=1C=C2C(C(NC2=CC1)=O)(C)C.[N+](=O)([O-])C=1C=C(C=CC1)B(O)O.C([O-])([O-])=O.[K+].[K+]>>CC1(C(NC2=CC=C(C=C12)C1=CC(=CC=C1)[N+](=O)[O-])=O)C
Br[c:10]1[cH:9][cH:8][c:7]2[c:21]([cH:20]1)[C:2]([CH3:1])([CH3:3])[C:4](=[O:5])[NH:6]2.OB(O)[c:11]1[cH:12][cH:13][cH:14][c:15]([N+:16](=[O:17])[O-:18])[cH:19]1>>[CH3:1][C:2]1([CH3:3])[C:4](=[O:5])[NH:6][c:7]2[cH:8][cH:9][c:10](-[c:11]3[cH:12][cH:13][cH:14][c:15]([N+:16](=[O:17])[O-:18])[cH:19]3)[cH:20][c:21]21
CC1(C)C(=O)Nc2ccc(Br)cc21.O=[N+]([O-])c1cccc(B(O)O)c1
CC1(C)C(=O)Nc2ccc(-c3cccc([N+](=O)[O-])c3)cc21
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
CCOC(=O)C.O.C(OC)COC
C-C Coupling
Suzuki coupling with boronic acids
9791290dea007c134587598bd16674eb122eb7281e427c61b6d8f55d72a5f584
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Cc2cc(-c3ccccc3)ccc2N1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:8]:[c:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9]:[c:10]
119
[{"value": 67.0, "product": "CC1(C(NC2=CC=C(C=C12)C1=CC(=CC=C1)[N+](=O)[O-])=O)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 119.0, "product": "CC1(C(NC2=CC=C(C=C12)C1=CC(=CC=C1)[N+](=O)[O-])=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
5-bromo-1,3-dihydro-3,3-dimethyl-2H-indol-2-one (1.02 g, 4.26 mmol) and tetrakis(triphenylphosphine)palladium(0) (0.244 g) were stirred under an atmosphere of nitrogen in dimethoxyethane (35 cm3). After 15 minutes, 3-nitrophenylboronic acid (1.43 g, 2.56 mmol) was added, followed by potassium carbonate (3.54 g, 2.56 mm...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2c(c1)CCN2.c1ccccc1
c1ccc2c(c1)CCN2.c1ccccc1
c1ccc2c(c1)CCN2.c1ccccc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.CCOC(=O)C.O.C(OC)COC
null
0.25
CC1(C)C(=O)Nc2ccc(Br)cc21.O=[N+]([O-])c1cccc(B(O)O)c1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.CCOC(=O)C.O.C(OC)COC>CC1(C)C(=O)Nc2ccc(-c3cccc([N+](=O)[O-])c3)cc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-1ed7f37270af420fb0e5d51ef1f37326
CCI.O=C1Cc2ccccc2N1>>CCC1=c2ccccc2=NC1=O
ICC.N1C(CC2=CC=CC=C12)=O.C(CCC)[Li].[NH4+].[Cl-].CN(CCN(C)C)C>>C(C)C=1C(N=C2C=CC=CC12)=O
I[CH2:2][CH3:1].[CH2:3]1[c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2[NH:10][C:11]1=[O:12]>>[CH3:1][CH2:2][C:3]1=[c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2=[N:10][C:11]1=[O:12]
CCI.O=C1Cc2ccccc2N1
CCC1=c2ccccc2=NC1=O
null
null
C1CCOC1
C-C Coupling
OtherReaction
7f8efd166912a03506850ad77dd8b310e9bbf110f40dc0aa3466aad53303d70b
9795126e672adf3dfeb9ebcd165d02e10eb1b4ac31d83997fdca7c7a739d39dc
O=C1C=c2ccccc2=N1
I-[CH2;D2;+0:1]-[C;D1;H3:2].[O;D1;H0:3]=[C:4]1-[CH2;D2;+0:5]-[c;H0;D3;+0:6]2:[c:7]:[c:8]:[c:9]:[c:10]:[c;H0;D3;+0:11]:2-[NH;D2;+0:12]-1>>[C;D1;H3:2]-[CH2;D2;+0:1]-[C;H0;D3;+0:5]1=[c;H0;D3;+0:6]2:[c:7]:[c:8]:[c:9]:[c:10]:[c;H0;D3;+0:11]:2=[N;H0;D2;+0:12]-[C:4]-1=[O;D1;H0:3]
2.9
[{"value": 2.9, "product": "C(C)C=1C(N=C2C=CC=CC12)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of oxindole (40 g, 0.3 mol) in dry THF (400 ml) under N2 was cooled to −25° C. and treated drop wise with n-butyl lithium (2.5M in hexanes, 240 ml, 0.6 mol). To the resulting solution was added N,N,N′,N′-tetramethylethylenediamine (90.4 ml, 0.6 mol). After 30 min. iodoethane (48 ml, 0.6 mol) was added and th...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Secondary amide
null
c1ccc2c(c1)CCN2
C1=c2ccccc2=NC1
C1=c2ccccc2=NC1
HI
C1CCOC1
null
null
CCI.O=C1Cc2ccccc2N1>C1CCOC1>CCC1=c2ccccc2=NC1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-a7d68ef0a88f48f89e4a0c15da7d1571
BrBr.CCC1C(=O)Nc2ccccc21>>CCC1C(=O)Nc2ccc(Br)cc21
C(C)C1C(NC2=CC=CC=C12)=O.C(C)(=O)[O-].[Na+].BrBr>>BrC=1C=C2C(C(NC2=CC1)=O)CC
Br[Br:11].[CH3:1][CH2:2][CH:3]1[C:4](=[O:5])[NH:6][c:7]2[cH:8][cH:9][cH:10][cH:12][c:13]21>>[CH3:1][CH2:2][CH:3]1[C:4](=[O:5])[NH:6][c:7]2[cH:8][cH:9][c:10]([Br:11])[cH:12][c:13]21
BrBr.CCC1C(=O)Nc2ccccc21
CCC1C(=O)Nc2ccc(Br)cc21
null
null
O.C(C)(=O)O
Functional Group Interconversion
Bromination
e5aad40fc3ec640bed45a7119ff569558b20c39979304f365dafdbc5ae4e4cd4
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
O=C1Cc2ccccc2N1
Br-[Br;H0;D1;+0:1].[c:2]:[c:3]:[cH;D2;+0:4]:[c:5]:[c:6]>>[Br;H0;D1;+0:1]-[c;H0;D3;+0:4](:[c:3]:[c:2]):[c:5]:[c:6]
null
[]
null
null
null
null
A solution of 3-ethyloxindole (6.0 g, 40 mmol) and sodium acetate (4 g, 48 mmol) in acetic acid (100 ml) was treated with bromine (6.4 g, 40 mmol). After 30 min. the mixture was diluted with water and extracted with EtOAc (2×); the combined organic layers were washed with water, sat. sodium hydrogen carbonate solution,...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2c(c1)CCN2
c1ccc2c(c1)CCN2
c1ccc2c(c1)CCN2
HBr
O.C(C)(=O)O
null
null
BrBr.CCC1C(=O)Nc2ccccc21>O.C(C)(=O)O>CCC1C(=O)Nc2ccc(Br)cc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-099a937005364924bd6eae4d9b0b8422
BrBr.CCC1(CC)C(=O)Nc2ccccc21>>CCC1(CC)C(=O)Nc2ccc(Br)cc21
C(C)C1(C(NC2=CC=CC=C12)=O)CC.C(C)(=O)[O-].[Na+].BrBr>>BrC=1C=C2C(C(NC2=CC1)=O)(CC)CC
Br[Br:13].[CH3:1][CH2:2][C:3]1([CH2:4][CH3:5])[C:6](=[O:7])[NH:8][c:9]2[cH:10][cH:11][cH:12][cH:14][c:15]21>>[CH3:1][CH2:2][C:3]1([CH2:4][CH3:5])[C:6](=[O:7])[NH:8][c:9]2[cH:10][cH:11][c:12]([Br:13])[cH:14][c:15]21
BrBr.CCC1(CC)C(=O)Nc2ccccc21
CCC1(CC)C(=O)Nc2ccc(Br)cc21
null
null
O.C(C)(=O)O
Functional Group Interconversion
Bromination
e5aad40fc3ec640bed45a7119ff569558b20c39979304f365dafdbc5ae4e4cd4
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
O=C1Cc2ccccc2N1
Br-[Br;H0;D1;+0:1].[c:2]:[c:3]:[cH;D2;+0:4]:[c:5]:[c:6]>>[Br;H0;D1;+0:1]-[c;H0;D3;+0:4](:[c:3]:[c:2]):[c:5]:[c:6]
null
[]
null
null
null
null
A solution of 3,3-diethylindol-2-one (8 g, 40 mmol) and sodium acetate (4 g, 48 mmol) in acetic acid (100 ml) was treated with bromine (6.4 g, 40 mmol). After 30 min. the mixture was diluted with water and extracted with EtOAc (2×); the combined organic layers were washed with water, sat. sodium hydrogen carbonate solu...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2c(c1)CCN2
c1ccc2c(c1)CCN2
c1ccc2c(c1)CCN2
HBr
O.C(C)(=O)O
null
null
BrBr.CCC1(CC)C(=O)Nc2ccccc21>O.C(C)(=O)O>CCC1(CC)C(=O)Nc2ccc(Br)cc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-685d956059c54290a7022e11e3dec19f
O=C1Nc2ccc(Br)cc2C1=O>>CC1(O)C(=O)Nc2ccc(Br)cc21
BrC=1C=C2C(C(NC2=CC1)=O)=O.C[Mg]Br.[Cl-].[NH4+]>>BrC=1C=C2C(C(NC2=CC1)=O)(C)O
[C:2]1(=[O:3])[C:4](=[O:5])[NH:6][c:7]2[cH:8][cH:9][c:10]([Br:11])[cH:12][c:13]21>>[CH3:1][C:2]1([OH:3])[C:4](=[O:5])[NH:6][c:7]2[cH:8][cH:9][c:10]([Br:11])[cH:12][c:13]21
O=C1Nc2ccc(Br)cc2C1=O
CC1(O)C(=O)Nc2ccc(Br)cc21
null
null
C1CCOC1
Miscellaneous
OtherReaction
e206534f58e7b072db5c84f71beb0f8b81df4661d962843e524e4fc82e2a18c5
8811b4d793f7cfa9f0f1f47a008648edabb54f371f76dfa680dd5b2e1564c6c5
O=C1Cc2ccccc2N1
[O;D1;H0:1]=[C:2]1-[#7:3]-[c:4]:[c:5](:[c:6])-[C;H0;D3;+0:7]-1=[O;H0;D1;+0:8]>>[C;D1;H3:9]-[C;H0;D4;+0:7]1(-[OH;D1;+0:8])-[C:2](=[O;D1;H0:1])-[#7:3]-[c:4]:[c:5]-1:[c:6]
29
[{"value": 29.0, "product": "BrC=1C=C2C(C(NC2=CC1)=O)(C)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 28.7, "product": "BrC=1C=C2C(C(NC2=CC1)=O)(C)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 5-bromoisatin (5.0 g, 22 mmol) in dry THF (50 cm3) under N2 was cooled to 0° C. and treated drop-wise with methyl magnesium bromide (3M in diethylether, 14.7 cm3, 44 mmol) and the mixture was allowed to warm up-to room temperature. The reaction was poured into sat. ammonium chloride solution, then extract...
10.6084/m9.figshare.5104873.v1
null
Ketone
Tertiary alcohol
c1ccc2c(c1)CCN2
c1ccc2c(c1)CCN2
c1ccc2c(c1)CCN2
Other
C1CCOC1
null
null
O=C1Nc2ccc(Br)cc2C1=O>C1CCOC1>CC1(O)C(=O)Nc2ccc(Br)cc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-a4bc0c246c5c49f69c45dc9f684b7b07
CC1(O)C(=O)Nc2ccc(Br)cc21.COS(=O)(=O)c1ccc(C)cc1>>COC1(C)C(=O)Nc2ccc(Br)cc21
[Cl-].[NH4+].CC(C)([O-])C.[K+].BrC=1C=C2C(C(NC2=CC1)=O)(C)O.COS(=O)(=O)C1=CC=C(C=C1)C>>BrC=1C=C2C(C(NC2=CC1)=O)(C)OC
[OH:2][C:3]1([CH3:4])[C:5](=[O:6])[NH:7][c:8]2[cH:9][cH:10][c:11]([Br:12])[cH:13][c:14]21.Cc1ccc(S(=O)(=O)O[CH3:1])cc1>>[CH3:1][O:2][C:3]1([CH3:4])[C:5](=[O:6])[NH:7][c:8]2[cH:9][cH:10][c:11]([Br:12])[cH:13][c:14]21
CC1(O)C(=O)Nc2ccc(Br)cc21.COS(=O)(=O)c1ccc(C)cc1
COC1(C)C(=O)Nc2ccc(Br)cc21
null
null
CN(C)C=O
Heteroatom Alkylation and Arylation
O-methylation
6e2efd44e881e9405bbc2be63bf815d40117fbb9fa6dc2effac725e566998d9a
81d2e2c5cd7c0d967284864f20b2202e3b06dde03416092c701808131566c9f8
O=C1Cc2ccccc2N1
C-c1:c:c:c(-S(=O)(=O)-O-[CH3;D1;+0:1]):c:c:1.[C;D1;H3:2]-[C:3]1(-[OH;D1;+0:4])-[c:5]:[c:6]-[#7:7]-[C:8]-1=[O;D1;H0:9]>>[C;D1;H3:2]-[C:3]1(-[O;H0;D2;+0:4]-[CH3;D1;+0:1])-[c:5]:[c:6]-[#7:7]-[C:8]-1=[O;D1;H0:9]
53.7
[{"value": 53.0, "product": "BrC=1C=C2C(C(NC2=CC1)=O)(C)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 53.7, "product": "BrC=1C=C2C(C(NC2=CC1)=O)(C)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
0
CELSIUS
null
null
5-bromo-3-hydroxy-3-methyl-1,3-dihydro-indol-2-one (1.0 g, 4.1 mmol) was dissolved in dry DMF (15 cm3) cooled to 0° C. and treated with potassium tert-butoxide (1M in THF, 4.5 cm3, 4.5 mmol). After 15 min. methyl-p-toluenesulfonate (0.93 g, 5 mmol) was added and the mixture was allowed to warm up-to room temperature. A...
10.6084/m9.figshare.5104873.v1
null
Tosylate.Tertiary alcohol
Ether
c1ccccc1
null
c1ccc2c(c1)CCN2
TsOH.HO-
CN(C)C=O
0
null
CC1(O)C(=O)Nc2ccc(Br)cc21.COS(=O)(=O)c1ccc(C)cc1>CN(C)C=O>COC1(C)C(=O)Nc2ccc(Br)cc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-ae65edd3a66e4dce8e06b975bf92e269
COC1(C)C(=O)Nc2ccc(Br)cc21.OB(O)c1cccc(Cl)c1>>COC1(C)C(=O)Nc2ccc(-c3cccc(Cl)c3)cc21
ClC=1C=C(C=CC1)B(O)O.C([O-])([O-])=O.[Na+].[Na+].BrC=1C=C2C(C(NC2=CC1)=O)(C)OC>>ClC=1C=C(C=CC1)C=1C=C2C(C(NC2=CC1)=O)(C)OC
Br[c:11]1[cH:10][cH:9][c:8]2[c:20]([cH:19]1)[C:3]([O:2][CH3:1])([CH3:4])[C:5](=[O:6])[NH:7]2.OB(O)[c:12]1[cH:13][cH:14][cH:15][c:16]([Cl:17])[cH:18]1>>[CH3:1][O:2][C:3]1([CH3:4])[C:5](=[O:6])[NH:7][c:8]2[cH:9][cH:10][c:11](-[c:12]3[cH:13][cH:14][cH:15][c:16]([Cl:17])[cH:18]3)[cH:19][c:20]21
COC1(C)C(=O)Nc2ccc(Br)cc21.OB(O)c1cccc(Cl)c1
COC1(C)C(=O)Nc2ccc(-c3cccc(Cl)c3)cc21
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.C(OC)COC
C-C Coupling
Suzuki coupling with boronic acids
9791290dea007c134587598bd16674eb122eb7281e427c61b6d8f55d72a5f584
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Cc2cc(-c3ccccc3)ccc2N1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:8]:[c:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9]:[c:10]
29
[{"value": 29.0, "product": "ClC=1C=C(C=CC1)C=1C=C2C(C(NC2=CC1)=O)(C)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 29.0, "product": "ClC=1C=C(C=CC1)C=1C=C2C(C(NC2=CC1)=O)(C)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
A solution of 5-bromo-3-methoxy-3-methyl-1,3-dihydro-indol-2-one (0.52 g, 2.0 mmol) and tetrakis(triphenylphosphine)palladium(0) (0.12 g, 0.1 mmol) was dissolved in dimethoxyethane (22 cm3). After 15 min., 3-chlorophenylboronic acid (0.63 g, 4.1 mmol) and sodium carbonate (1.0 g) in water (10 cm3) was added and the rea...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2c(c1)CCN2.c1ccccc1
c1ccc2c(c1)CCN2.c1ccccc1
c1ccc2c(c1)CCN2.c1ccccc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.C(OC)COC
null
0.25
COC1(C)C(=O)Nc2ccc(Br)cc21.OB(O)c1cccc(Cl)c1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.C(OC)COC>COC1(C)C(=O)Nc2ccc(-c3cccc(Cl)c3)cc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-11c8f6a6d49c4e53ba77cc33793f0bd3
CC#[C][Mg][Br].O=C1Nc2ccc(Br)cc2C1=O>>CC#CC1(O)C(=O)Nc2ccc(Br)cc21
[Cl-].[NH4+].BrC=1C=C2C(C(NC2=CC1)=O)=O.C(#CC)[Mg]Br>>BrC=1C=C2C(C(NC2=CC1)=O)(C#CC)O
[Br][Mg][C:3]#[C:2][CH3:1].[C:4]1(=[O:5])[C:6](=[O:7])[NH:8][c:9]2[cH:10][cH:11][c:12]([Br:13])[cH:14][c:15]21>>[CH3:1][C:2]#[C:3][C:4]1([OH:5])[C:6](=[O:7])[NH:8][c:9]2[cH:10][cH:11][c:12]([Br:13])[cH:14][c:15]21
CC#[C][Mg][Br].O=C1Nc2ccc(Br)cc2C1=O
CC#CC1(O)C(=O)Nc2ccc(Br)cc21
null
null
C1CCOC1
C-C Coupling
Grignard from ketone to alcohol
047bdb50f80bc54c741bf0904b2597c43eb1b755af59b6d94feb30812db22dae
14e780921369c95ed40af45076e892db051e7adf9725dbd330196dcdac285701
O=C1Cc2ccccc2N1
[Br]-[Mg]-[C;H0;D2;+0:1]#[C:2]-[C;D1;H3:3].[O;D1;H0:4]=[C:5]1-[#7:6]-[c:7]:[c:8](:[c:9])-[C;H0;D3;+0:10]-1=[O;H0;D1;+0:11]>>[C;D1;H3:3]-[C:2]#[C;H0;D2;+0:1]-[C;H0;D4;+0:10]1(-[OH;D1;+0:11])-[C:5](=[O;D1;H0:4])-[#7:6]-[c:7]:[c:8]-1:[c:9]
97
[{"value": 97.0, "product": "BrC=1C=C2C(C(NC2=CC1)=O)(C#CC)O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 96.4, "product": "BrC=1C=C2C(C(NC2=CC1)=O)(C#CC)O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
To a solution of 5-bromoisatin (2.5 g, 11 mmol) in dry THF (100 cm3) at −10° C. under a nitrogen atmosphere was added 1-propynylmagnesium bromide (0.5 M in THF, 47 cm3, 23.5 mmol). After 1 h, the mixture was poured into saturated ammonium chloride and extracted with EtOAc (×3), washed with brine, dried (MgSO4) and evap...
10.6084/m9.figshare.5104873.v1
null
Magnesium halide.Ketone.Alkyne
Tertiary alcohol.Alkyne
c1ccc2c(c1)CCN2
c1ccc2c(c1)CCN2
c1ccc2c(c1)CCN2
Br-.Mg
C1CCOC1
null
1
CC#[C][Mg][Br].O=C1Nc2ccc(Br)cc2C1=O>C1CCOC1>CC#CC1(O)C(=O)Nc2ccc(Br)cc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-26adb8c2c647457e80fdfa7a30ae1c31
CC#CC1(OC)C(=O)Nc2ccc(Br)cc21.OB(O)c1cccc(Cl)c1>>CC#CC1(OC)C(=O)Nc2ccc(-c3cccc(Cl)c3)cc21
ClC=1C=C(C=CC1)B(O)O.C([O-])([O-])=O.[Na+].[Na+].BrC=1C=C2C(C(NC2=CC1)=O)(C#CC)OC>>ClC=1C=C(C=CC1)C=1C=C2C(C(NC2=CC1)=O)(C#CC)OC
Br[c:13]1[cH:12][cH:11][c:10]2[c:22]([cH:21]1)[C:4]([C:3]#[C:2][CH3:1])([O:5][CH3:6])[C:7](=[O:8])[NH:9]2.OB(O)[c:14]1[cH:15][cH:16][cH:17][c:18]([Cl:19])[cH:20]1>>[CH3:1][C:2]#[C:3][C:4]1([O:5][CH3:6])[C:7](=[O:8])[NH:9][c:10]2[cH:11][cH:12][c:13](-[c:14]3[cH:15][cH:16][cH:17][c:18]([Cl:19])[cH:20]3)[cH:21][c:22]21
CC#CC1(OC)C(=O)Nc2ccc(Br)cc21.OB(O)c1cccc(Cl)c1
CC#CC1(OC)C(=O)Nc2ccc(-c3cccc(Cl)c3)cc21
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.C(OC)COC
C-C Coupling
Suzuki coupling with boronic acids
9791290dea007c134587598bd16674eb122eb7281e427c61b6d8f55d72a5f584
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Cc2cc(-c3ccccc3)ccc2N1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:3]:[c:2]:[c;H0;D3;+0:1](-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]):[c:4]:[c:5]
15
[{"value": 15.0, "product": "ClC=1C=C(C=CC1)C=1C=C2C(C(NC2=CC1)=O)(C#CC)OC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 15.0, "product": "ClC=1C=C(C=CC1)C=1C=C2C(C(NC2=CC1)=O)(C#CC)OC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
5-bromo-3-methoxy-3-prop-1-ynyl-1,3-dihydroindol-2-one (0.56 g, 2.0 mmol) and tetrakis(triphenylphosphine)palladium(0) (0.12 g, 0.10 mmol) were stirred at room temperature in dimethoxyethane (22 cm3). After 15 min. 3-chlorophenylboronic acid (0.63 g, 4.0 mmol) and sodium carbonate (1.06 g, 10 mmol) in water (11 cm3) we...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2c(c1)CCN2.c1ccccc1
c1ccc2c(c1)CCN2.c1ccccc1
c1ccc2c(c1)CCN2.c1ccccc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.C(OC)COC
null
0.25
CC#CC1(OC)C(=O)Nc2ccc(Br)cc21.OB(O)c1cccc(Cl)c1>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.C(OC)COC>CC#CC1(OC)C(=O)Nc2ccc(-c3cccc(Cl)c3)cc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-c09160befb0a446b9eccd6a4f009836e
O=C1Cc2cc(Br)ccc2N1.OB(O)c1cccc(Cl)c1>>O=C1Cc2cc(-c3cccc(Cl)c3)ccc2N1
BrC=1C=C2CC(NC2=CC1)=O.ClC=1C=C(C=CC1)B(O)O.C([O-])([O-])=O.[Na+].[Na+]>>ClC=1C=C(C=CC1)C=1C=C2CC(NC2=CC1)=O
Br[c:6]1[cH:5][c:4]2[c:16]([cH:15][cH:14]1)[NH:17][C:2](=[O:1])[CH2:3]2.OB(O)[c:7]1[cH:8][cH:9][cH:10][c:11]([Cl:12])[cH:13]1>>[O:1]=[C:2]1[CH2:3][c:4]2[cH:5][c:6](-[c:7]3[cH:8][cH:9][cH:10][c:11]([Cl:12])[cH:13]3)[cH:14][cH:15][c:16]2[NH:17]1
O=C1Cc2cc(Br)ccc2N1.OB(O)c1cccc(Cl)c1
O=C1Cc2cc(-c3cccc(Cl)c3)ccc2N1
null
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1
O.C(OC)COC
C-C Coupling
Suzuki coupling with boronic acids
9791290dea007c134587598bd16674eb122eb7281e427c61b6d8f55d72a5f584
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Cc2cc(-c3ccccc3)ccc2N1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:8]:[c:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9]:[c:10]
86
[{"value": 86.0, "product": "ClC=1C=C(C=CC1)C=1C=C2CC(NC2=CC1)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 83.3, "product": "ClC=1C=C(C=CC1)C=1C=C2CC(NC2=CC1)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of the 5-bromoxindole (0.5 g, 2.4 mmol) and tetrakis(triphenylphosphine) palladium (0.14 g, 0.12 mmol) in dimethoxyethane (10 cm3) was stirred under N2 for 20 min. To this mixture was then added 3-chlorophenylboronic acid (0.44 g, 2.83 mmol) and sodium carbonate (0.75 g, 7.1 mmol) in water (4 cm3). The solut...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2c(c1)CCN2.c1ccccc1
c1ccc2c(c1)CCN2.c1ccccc1
c1ccc2c(c1)CCN2.c1ccccc1
HBr.B
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.O.C(OC)COC
null
null
O=C1Cc2cc(Br)ccc2N1.OB(O)c1cccc(Cl)c1>[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.O.C(OC)COC>O=C1Cc2cc(-c3cccc(Cl)c3)ccc2N1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-eb6667c882384f968c20f1307ce31ead
O=C1Cc2cc(-c3cccc(Cl)c3)ccc2N1>>O=C1Nc2ccc(-c3cccc(Cl)c3)cc2C1=O
ClC=1C=C(C=CC1)C=1C=C2CC(NC2=CC1)=O.O1CCOCC1>>ClC=1C=C(C=CC1)C=1C=C2C(C(NC2=CC1)=O)=O
[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][c:7](-[c:8]3[cH:9][cH:10][cH:11][c:12]([Cl:13])[cH:14]3)[cH:15][c:16]2[CH2:17]1>>[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][c:7](-[c:8]3[cH:9][cH:10][cH:11][c:12]([Cl:13])[cH:14]3)[cH:15][c:16]2[C:17]1=[O:18]
O=C1Cc2cc(-c3cccc(Cl)c3)ccc2N1
O=C1Nc2ccc(-c3cccc(Cl)c3)cc2C1=O
null
null
null
Oxidation
OtherReaction
5c42bc08649ad444bd707dcd6481bf7bab42c2368ef82c0ac85a3860aab46162
77bee5a21cba7564f2a068b8a8fb160e4513dc5cbafb6b06748cb7a2efc1051b
O=C1Nc2ccc(-c3ccccc3)cc2C1=O
[O;D1;H0:1]=[C:2]1-[#7:3]-[c:4]:[c:5](:[c:6])-[CH2;D2;+0:7]-1>>[O;D1;H0:8]=[C;H0;D3;+0:7]1-[C:2](=[O;D1;H0:1])-[#7:3]-[c:4]:[c:5]-1:[c:6]
76
[{"value": 76.0, "product": "ClC=1C=C(C=CC1)C=1C=C2C(C(NC2=CC1)=O)=O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 5-(3-Chloro-phenyl)-1,3-dihydro-indol-2-one (10.0 g, 41 mmol) in dioxane (200 cm3) and SeO2 (22.8 g, 205 mmol) was brought to reflux for 2 h then cooled to RT and concentrated onto Florisil. The Florisil was washed (acetone:CHCl3 1:9) and the combined organic extracts were evaporated. The residue was puri...
10.6084/m9.figshare.5104873.v1
null
null
Ketone
c1ccc2c(c1)CCN2
c1ccc2c(c1)CCN2
c1ccc2c(c1)CCN2.c1ccccc1
Other
null
null
null
O=C1Cc2cc(-c3cccc(Cl)c3)ccc2N1>>O=C1Nc2ccc(-c3cccc(Cl)c3)cc2C1=O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-0951505fdd3d4c26a4e8069af7835193
ICCCCI.O=C1Cc2ccccc2N1>>O=C1Nc2ccccc2C12CCCC2
N1C(CC2=CC=CC=C12)=O.C(CCC)[Li].ICCCCI.CN(CCN(C)C)C>>N1C(C2(C3=CC=CC=C13)CCCC2)=O
I[CH2:11][CH2:12][CH2:13][CH2:14]I.[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2[CH2:10]1>>[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2[C:10]12[CH2:11][CH2:12][CH2:13][CH2:14]2
ICCCCI.O=C1Cc2ccccc2N1
O=C1Nc2ccccc2C12CCCC2
null
null
C1CCOC1.O
C-C Coupling
OtherReaction
da305b19e438cec6dd9ecd353ca3cd934886dd4c5b3846022dac2a623fceb79e
7b68950fc1047c59bb49c25e850f5a51cbe91a99bb87839c4547aec123110e4b
O=C1Nc2ccccc2C12CCCC2
I-[CH2;D2;+0:1]-[C:2]-[C:3]-[CH2;D2;+0:4]-I.[O;D1;H0:5]=[C:6]1-[#7:7]-[c:8]:[c:9](:[c:10])-[CH2;D2;+0:11]-1>>[O;D1;H0:5]=[C:6]1-[#7:7]-[c:8]:[c:9](:[c:10])-[C;H0;D4;+0:11]-12-[CH2;D2;+0:1]-[C:2]-[C:3]-[CH2;D2;+0:4]-2
50
[{"value": 50.0, "product": "N1C(C2(C3=CC=CC=C13)CCCC2)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 50.0, "product": "N1C(C2(C3=CC=CC=C13)CCCC2)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
14
HOUR
To a −25° C. solution of oxindole (2.0 g, 15.0 mmol) in 40 (cm3) of anhydrous THF under N2 was added n-butyllithium (1.6 M in hexanes, 19.7 cm3, 31.5 mmol) drop-wise. To the resulting milky solution was added N,N,N′,N′-tetramethylethylenediamine (4.75 cm3, 31.5 mmol). After 30 min. a solution of 1,4-diiodobutane (21.9 ...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary halide
null
c1ccc2c(c1)CCN2
c1ccc2c(c1)NCC21CCCC1
c1ccc2c(c1)NCC21CCCC1
HI
C1CCOC1.O
null
14
ICCCCI.O=C1Cc2ccccc2N1>C1CCOC1.O>O=C1Nc2ccccc2C12CCCC2
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-b5f70c65da144f20b845befc93cdc22b
BrBr.O=C1Nc2ccccc2C12CCCC2>>O=C1Nc2ccccc2C12CCCC2Br
C(O)([O-])=O.[Na+].N1C(C2(C3=CC=CC=C13)CCCC2)=O.C(C)(=O)[O-].[Na+].BrBr>>BrC1CCCC12C(NC1=CC=CC=C21)=O
Br[Br:15].[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2[C:10]12[CH2:11][CH2:12][CH2:13][CH2:14]2>>[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2[C:10]12[CH2:11][CH2:12][CH2:13][CH:14]2[Br:15]
BrBr.O=C1Nc2ccccc2C12CCCC2
O=C1Nc2ccccc2C12CCCC2Br
null
null
C(C)(=O)O
Functional Group Interconversion
Bromination
5d1ae453742bff017caef24079c4e11e210e4fe7fcd315c0a1d757dce473ae36
0c353a1260488c22c3ffb72de5623420c3ec35470a0b3a2045b11c29224f458e
O=C1Nc2ccccc2C12CCCC2
Br-[Br;H0;D1;+0:1].[O;D1;H0:2]=[C:3]1-[#7:4]-[c:5]:[c:6]-[C:7]-12-[C:8]-[C:9]-[C:10]-[CH2;D2;+0:11]-2>>[Br;H0;D1;+0:1]-[CH;D3;+0:11]1-[C:10]-[C:9]-[C:8]-[C:7]-12-[c:6]:[c:5]-[#7:4]-[C:3]-2=[O;D1;H0:2]
105
[{"value": 96.0, "product": "BrC1CCCC12C(NC1=CC=CC=C21)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 105.0, "product": "BrC1CCCC12C(NC1=CC=CC=C21)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of spiro[cyclopentane-1,3′-[3H]indol]-2′(1′H)-one (0.27 g, 1.4 mmol) and sodium acetate (0.12 g, 1.46 mmol) in acetic acid (10 cm3) was treated with bromine (0.24 g, 1.51 mmol) in acetic acid (2 cm3). After 30 min. the mixture was poured into sat. sodium hydrogen carbonate solution and extracted with EtOAc (...
10.6084/m9.figshare.5104873.v1
null
null
Secondary halide
c1ccc2c(c1)NCC21CCCC1
c1ccc2c(c1)NCC21CCCC1
c1ccc2c(c1)NCC21CCCC1
HBr
C(C)(=O)O
null
null
BrBr.O=C1Nc2ccccc2C12CCCC2>C(C)(=O)O>O=C1Nc2ccccc2C12CCCC2Br
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-d24153be9c474bb28c86121b580a0c0d
ICCCCCI.O=C1Cc2ccccc2N1>>O=C1Nc2ccccc2C12CCCCC2
ICCCCCI.N1C(CC2=CC=CC=C12)=O.C(CCC)[Li].[Cl-].[NH4+].CN(CCN(C)C)C>>N1C(C2(C3=CC=CC=C13)CCCCC2)=O
I[CH2:11][CH2:12][CH2:13][CH2:14][CH2:15]I.[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2[CH2:10]1>>[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2[C:10]12[CH2:11][CH2:12][CH2:13][CH2:14][CH2:15]2
ICCCCCI.O=C1Cc2ccccc2N1
O=C1Nc2ccccc2C12CCCCC2
null
null
CCOC(=O)C.O1CCCC1
C-C Coupling
OtherReaction
579f0f36d3c1f227acfe012179441842108aef707a45bbf7908129260433618c
7b68950fc1047c59bb49c25e850f5a51cbe91a99bb87839c4547aec123110e4b
O=C1Nc2ccccc2C12CCCCC2
I-[CH2;D2;+0:1]-[C:2]-[C:3]-[C:4]-[CH2;D2;+0:5]-I.[O;D1;H0:6]=[C:7]1-[#7:8]-[c:9]:[c:10](:[c:11])-[CH2;D2;+0:12]-1>>[O;D1;H0:6]=[C:7]1-[#7:8]-[c:9]:[c:10](:[c:11])-[C;H0;D4;+0:12]-12-[CH2;D2;+0:1]-[C:2]-[C:3]-[C:4]-[CH2;D2;+0:5]-2
69.6
[{"value": 69.6, "product": "N1C(C2(C3=CC=CC=C13)CCCCC2)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 68.8, "product": "N1C(C2(C3=CC=CC=C13)CCCCC2)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
15
MINUTE
A solution of oxindole (25 g, 0.19 mol) in anhydrous tetrahydrofuran (800 cm3) was cooled to −20° C., then n-butyllithium (2.5M in hexanes, 152 cm3, 0.38 mol) was added slowly followed by N,N,N′,N′-tetramethylethylenediamine (51 cm3, 0.38 mol,). After 15 min. 1,5-diiodopentane (174 g, 0.54 mol) was added slowly and the...
10.6084/m9.figshare.5104873.v1
null
Primary halide.Primary halide
null
c1ccc2c(c1)CCN2
c1ccc2c(c1)NCC21CCCCC1
c1ccc2c(c1)NCC21CCCCC1
HI
CCOC(=O)C.O1CCCC1
null
0.25
ICCCCCI.O=C1Cc2ccccc2N1>CCOC(=O)C.O1CCCC1>O=C1Nc2ccccc2C12CCCCC2
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-e265dcbe7a30486b9c3ee7c9ec1cbc9e
BrBr.O=C1Nc2ccccc2C12CCCCC2>>O=C1Nc2ccc(Br)cc2C12CCCCC2
N1C(C2(C3=CC=CC=C13)CCCCC2)=O.C(C)(=O)[O-].[Na+].BrBr>>BrC=1C=C2C3(C(NC2=CC1)=O)CCCCC3
Br[Br:8].[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][cH:7][cH:9][c:10]2[C:11]12[CH2:12][CH2:13][CH2:14][CH2:15][CH2:16]2>>[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][c:7]([Br:8])[cH:9][c:10]2[C:11]12[CH2:12][CH2:13][CH2:14][CH2:15][CH2:16]2
BrBr.O=C1Nc2ccccc2C12CCCCC2
O=C1Nc2ccc(Br)cc2C12CCCCC2
null
null
C(C)(=O)O
Functional Group Interconversion
Bromination
b75a0cb1be6e87ac5ae2a0c4fc61b176231cdf76c6a5c5e00ef053906cd4efba
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
O=C1Nc2ccccc2C12CCCCC2
Br-[Br;H0;D1;+0:1].[c:2]:[c:3]:[cH;D2;+0:4]:[c:5]:[c:6]>>[Br;H0;D1;+0:1]-[c;H0;D3;+0:4](:[c:5]:[c:6]):[c:3]:[c:2]
67
[{"value": 67.0, "product": "BrC=1C=C2C3(C(NC2=CC1)=O)CCCCC3", "details": "PERCENTYIELD", "is_desired": false}, {"value": 65.4, "product": "BrC=1C=C2C3(C(NC2=CC1)=O)CCCCC3", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
To a solution of spiro[cyclohexane-1,3′-[3H]indol]-2′(1′H)-one (17.6 g, 0.09 mol) in acetic acid (300 cm3) was added sodium acetate (8.0 g, 0.1 mol) and bromine (14.6 g, 0.091 mol) with stirring. After 30 min. at room temperature, the reaction mixture was partitioned between water and EtOAc. The aqueous phase was extra...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2c(c1)NCC21CCCCC1
c1ccc2c(c1)NCC21CCCCC1
c1ccc2c(c1)NCC21CCCCC1
HBr
C(C)(=O)O
null
0.5
BrBr.O=C1Nc2ccccc2C12CCCCC2>C(C)(=O)O>O=C1Nc2ccc(Br)cc2C12CCCCC2
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-da0442915f5d4115aac6c6d518dc2906
CC(C)(C)OC(=O)n1cccc1B(O)O.O=C1Nc2ccc(Br)cc2C12CCCCC2>>CC(C)(C)OC(=O)n1cccc1-c1ccc2c(c1)C1(CCCCC1)C(=O)N2
B(O)(O)C=1N(C=CC1)C(=O)OC(C)(C)C.C(=O)([O-])[O-].[K+].[K+].BrC=1C=C2C3(C(NC2=CC1)=O)CCCCC3>>O=C1NC2=CC=C(C=C2C12CCCCC2)C=2N(C=CC2)C(=O)OC(C)(C)C
OB(O)[c:12]1[n:8]([C:6]([O:5][C:2]([CH3:1])([CH3:3])[CH3:4])=[O:7])[cH:9][cH:10][cH:11]1.Br[c:13]1[cH:14][cH:15][c:16]2[c:17]([cH:18]1)[C:19]1([CH2:20][CH2:21][CH2:22][CH2:23][CH2:24]1)[C:25](=[O:26])[NH:27]2>>[CH3:1][C:2]([CH3:3])([CH3:4])[O:5][C:6](=[O:7])[n:8]1[cH:9][cH:10][cH:11][c:12]1-[c:13]1[cH:14][cH:15][c:16]2...
CC(C)(C)OC(=O)n1cccc1B(O)O.O=C1Nc2ccc(Br)cc2C12CCCCC2
CC(C)(C)OC(=O)n1cccc1-c1ccc2c(c1)C1(CCCCC1)C(=O)N2
null
null
O
C-C Coupling
Suzuki coupling with boronic acids
72cb0722e2dfbd8433f7f279041b17208e2a10c7d719ed09e6c4b6dd1c93185b
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Nc2ccc(-c3ccc[nH]3)cc2C12CCCCC2
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6]1:[c:7]:[c:8]:[c:9]:[#7;a:10]:1-[C:11](=[O;D1;H0:12])-[#8:13]-[C:14](-[C;D1;H3:15])(-[C;D1;H3:16])-[C;D1;H3:17]>>[C;D1;H3:15]-[C:14](-[C;D1;H3:16])(-[C;D1;H3:17])-[#8:13]-[C:11](=[O;D1;H0:12])-[#7;a:10]1:[c:9]:[c:8]:[c:7]:[c;H0;D3;+0:6]:1-[c;H0;D3;+0:1](...
null
[]
80
CELSIUS
15
MINUTE
To a solution of 5′-bromo-spiro[cyclohexane-1,3′-indolin]-2′-one (3.4 g, 12 mmol) in 1,2-DME (100 mL) under a nitrogen atmosphere was added tetrakis(triphenylphospine)palladium(0) (70 mg, 5 mol %). After 15 min, 2-borono-1H-pyrrole-1-carboxylic acid, 1-tert butyl ester (1.3 eq, 3.31 g, 15.6 mmol) and a solution of K2CO...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc[nH]1.c1ccc2c(c1)NCC21CCCCC1
c1ccc[nH]1.c1ccc2c(c1)NCC21CCCCC1
c1ccc[nH]1.c1ccc2c(c1)NCC21CCCCC1
HBr.B
O
80
0.25
CC(C)(C)OC(=O)n1cccc1B(O)O.O=C1Nc2ccc(Br)cc2C12CCCCC2>O>CC(C)(C)OC(=O)n1cccc1-c1ccc2c(c1)C1(CCCCC1)C(=O)N2
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-8c3dd858b8414819a8fc99e075305940
CI.O=C1Nc2ccc(-c3ccc[nH]3)cc2C12CCCCC2>>Cn1cccc1-c1ccc2c(c1)C1(CCCCC1)C(=O)N2
O.N1C(=CC=C1)C=1C=C2C3(C(NC2=CC1)=O)CCCCC3.C([O-])([O-])=O.[K+].[K+].IC>>CN1C(=CC=C1)C=1C=C2C3(C(NC2=CC1)=O)CCCCC3
I[CH3:1].[nH:2]1[cH:3][cH:4][cH:5][c:6]1-[c:7]1[cH:8][cH:9][c:10]2[c:11]([cH:12]1)[C:13]1([CH2:14][CH2:15][CH2:16][CH2:17][CH2:18]1)[C:19](=[O:20])[NH:21]2>>[CH3:1][n:2]1[cH:3][cH:4][cH:5][c:6]1-[c:7]1[cH:8][cH:9][c:10]2[c:11]([cH:12]1)[C:13]1([CH2:14][CH2:15][CH2:16][CH2:17][CH2:18]1)[C:19](=[O:20])[NH:21]2
CI.O=C1Nc2ccc(-c3ccc[nH]3)cc2C12CCCCC2
Cn1cccc1-c1ccc2c(c1)C1(CCCCC1)C(=O)N2
null
null
CCOC(=O)C.CN(C)C=O
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
3b0bd5806650bb387428bf36a5e436078e57d40d2afdf9e751829e2a02da9e1d
7a358c636daddc97c1fb4c29f378044d7eac3f01815d9966e599841f642d631a
O=C1Nc2ccc(-c3ccc[nH]3)cc2C12CCCCC2
I-[CH3;D1;+0:1].[c:2]-[c:3]1:[c:4]:[c:5]:[c:6]:[nH;D2;+0:7]:1>>[CH3;D1;+0:1]-[n;H0;D3;+0:7]1:[c:6]:[c:5]:[c:4]:[c:3]:1-[c:2]
92.3
[{"value": 76.0, "product": "CN1C(=CC=C1)C=1C=C2C3(C(NC2=CC1)=O)CCCCC3", "details": "PERCENTYIELD", "is_desired": false}, {"value": 92.3, "product": "CN1C(=CC=C1)C=1C=C2C3(C(NC2=CC1)=O)CCCCC3", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
16
HOUR
A mixture of 5′-(1H-pyrrole-2-yl)spiro[cyclohexane-1,3′-[3H]indol]-2′(1′H)-one (0.46 g, 1.7 mmol) and potassium carbonate (5 eq, 1.18 g, 8.6 mmol) in DMF (2 mL) at room temperature was treated with a solution of iodomethane (3 eq, 0.32 g, 5.1 mmol) in DMF (1 mL). The solution was stirred 16 h at room temperature, then ...
10.6084/m9.figshare.5104873.v1
null
null
null
c1cc[nH]c1
c1ccc[nH]1
c1ccc[nH]1.c1ccc2c(c1)NCC21CCCCC1
HI
CCOC(=O)C.CN(C)C=O
null
16
CI.O=C1Nc2ccc(-c3ccc[nH]3)cc2C12CCCCC2>CCOC(=O)C.CN(C)C=O>Cn1cccc1-c1ccc2c(c1)C1(CCCCC1)C(=O)N2
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-9ecd93464dc648fe987299a1452499ec
CN(C)C=O.Fc1cc(Br)cc(Br)c1>>O=Cc1cc(F)cc(Br)c1
CN(C)C=O.BrC=1C=C(C=C(C1)Br)F.C(CCC)[Li]>>FC=1C=C(C=O)C=C(C1)Br
CN(C)[CH:2]=[O:1].Br[c:3]1[cH:4][c:5]([F:6])[cH:7][c:8]([Br:9])[cH:10]1>>[O:1]=[CH:2][c:3]1[cH:4][c:5]([F:6])[cH:7][c:8]([Br:9])[cH:10]1
CN(C)C=O.Fc1cc(Br)cc(Br)c1
O=Cc1cc(F)cc(Br)c1
null
null
C(C)OCC
C-C Coupling
Bouveault aldehyde synthesis
4664d189e1ff40b394aee0a7d0943c7bfc06c1f81f238cff6865649dda594153
afd09ced98f25d311f21cc04ba6a50fe7e5516de47e17484683ded13d323b1b2
c1ccccc1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].C-N(-C)-[CH;D2;+0:6]=[O;D1;H0:7]>>[O;D1;H0:7]=[CH;D2;+0:6]-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]
100
[{"value": 100.0, "product": "FC=1C=C(C=O)C=C(C1)Br", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
To a solution of 3,5-dibromofluorobenzene in diethyl ether (100 cm3) at −78° C. was added n-butyl lithium (2.5 M, 8 cm3, 20 mmol) dropwise. After 30 min. the mixture was treated with DMF (20 cm3) in diethyl ether (10 cm3) and stirring was continued at −78° C. After 30 min. the mixture was quenched with dilute HCl aq., ...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Tertiary amide
Aldehyde
c1ccccc1
c1ccccc1
c1ccccc1
HBr
C(C)OCC
null
null
CN(C)C=O.Fc1cc(Br)cc(Br)c1>C(C)OCC>O=Cc1cc(F)cc(Br)c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-127f208a746641c1877f78d37d4f625e
ON=Cc1cc(F)cc(Br)c1>>N#Cc1cc(F)cc(Br)c1
FC=1C=C(C=NO)C=C(C1)Br>>FC=1C=C(C#N)C=C(C1)Br
O[N:1]=[CH:2][c:3]1[cH:4][c:5]([F:6])[cH:7][c:8]([Br:9])[cH:10]1>>[N:1]#[C:2][c:3]1[cH:4][c:5]([F:6])[cH:7][c:8]([Br:9])[cH:10]1
ON=Cc1cc(F)cc(Br)c1
N#Cc1cc(F)cc(Br)c1
null
C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-]
C(C)#N
Functional Group Interconversion
OtherReaction
17f476cc256704e312f02cdb730538a4d2e78e129aaed9ef4aa555a9b052c890
9ad4e779dba60265752423413bc1b61ff9562539f91b24f3b3d9205e4bb46232
c1ccccc1
O-[N;H0;D2;+0:1]=[CH;D2;+0:2]-[c:3](:[c:4]):[c:5]>>[N;H0;D1;+0:1]#[C;H0;D2;+0:2]-[c:3](:[c:4]):[c:5]
89.3
[{"value": 89.0, "product": "FC=1C=C(C#N)C=C(C1)Br", "details": "PERCENTYIELD", "is_desired": false}, {"value": 89.3, "product": "FC=1C=C(C#N)C=C(C1)Br", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
5
HOUR
The above oxime (3.76 g, 17.24 mmol) and copper (II) acetate (370 mg) were dissolved in acetonitrile (100 cm3) under nitrogen and heated under reflux. After 5 h, the mixture was evaporated, the residue taken into EtOAc, washed with sulfuric acid (1N), water, brine, dried (MgSO4) and evaporated to give 3-fluoro-5-bromob...
10.6084/m9.figshare.5104873.v1
null
Oxime
Nitrile
null
null
c1ccccc1
HO-
C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-].C(C)#N
null
5
ON=Cc1cc(F)cc(Br)c1>C(C)(=O)[O-].[Cu+2].C(C)(=O)[O-].C(C)#N>N#Cc1cc(F)cc(Br)c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-bb177ac4f5ee408d9791a43cc1ab2c73
CCOC(OCC)OCC.N#Cc1cc(F)cc(-c2ccc3c(c2)C2(CCCCC2)C(=O)N3)c1>>CCOC(OCC)N1C(=O)C2(CCCCC2)c2cc(-c3cc(F)cc(C#N)c3)ccc21
O=C1NC2=CC=C(C=C2C12CCCCC2)C=2C=C(C#N)C=C(C2)F.C(C)OC(OCC)OCC>>C(C)OC(N1C(C2(C3=CC(=CC=C13)C=1C=C(C#N)C=C(C1)F)CCCCC2)=O)OCC
CCO[CH:4]([O:3][CH2:2][CH3:1])[O:5][CH2:6][CH3:7].[NH:8]1[C:9](=[O:10])[C:11]2([CH2:12][CH2:13][CH2:14][CH2:15][CH2:16]2)[c:17]2[cH:18][c:19](-[c:20]3[cH:21][c:22]([F:23])[cH:24][c:25]([C:26]#[N:27])[cH:28]3)[cH:29][cH:30][c:31]21>>[CH3:1][CH2:2][O:3][CH:4]([O:5][CH2:6][CH3:7])[N:8]1[C:9](=[O:10])[C:11]2([CH2:12][CH2:1...
CCOC(OCC)OCC.N#Cc1cc(F)cc(-c2ccc3c(c2)C2(CCCCC2)C(=O)N3)c1
CCOC(OCC)N1C(=O)C2(CCCCC2)c2cc(-c3cc(F)cc(C#N)c3)ccc21
null
null
null
Heteroatom Alkylation and Arylation
OtherReaction
f5b83fcf4b9c65194b6e5c49370fc988f96979e0bef62f46742babca4127b463
1ec70821ce282b2f30be459652d8181f281dba872707ca835b3678072970aef7
O=C1Nc2ccc(-c3ccccc3)cc2C12CCCCC2
C-C-O-[CH;D3;+0:1](-[#8:2]-[C:3])-[#8:4]-[C:5].[O;D1;H0:6]=[C:7]1-[C:8]-[c:9]:[c:10](:[c:11])-[NH;D2;+0:12]-1>>[C:3]-[#8:2]-[CH;D3;+0:1](-[#8:4]-[C:5])-[N;H0;D3;+0:12]1-[C:7](=[O;D1;H0:6])-[C:8]-[c:9]:[c:10]-1:[c:11]
56.4
[{"value": 56.0, "product": "C(C)OC(N1C(C2(C3=CC(=CC=C13)C=1C=C(C#N)C=C(C1)F)CCCCC2)=O)OCC", "details": "PERCENTYIELD", "is_desired": false}, {"value": 56.4, "product": "C(C)OC(N1C(C2(C3=CC(=CC=C13)C=1C=C(C#N)C=C(C1)F)CCCCC2)=O)OCC", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 3-(1′,2′-dihydro-2′-oxospiro[cyclohexane-1,3′-[3H]indol]-5′-yl)-5-flurobenzonitrile (1.0 eq, 0.27 g, 0.84 mmol) in triethylorthoformate (2 mL, 12 mmol) was heated to 150° C. for 1 h. The reaction mixture was allowed to cool, the excess triethylorthoformate was removed in vacuo, and the residue was purifie...
10.6084/m9.figshare.5104873.v1
null
Ether.Ether.Ether.Secondary amide
Ether.Ether.Tertiary amide
c1ccc2c(c1)NCC21CCCCC1
c1ccc2c(c1)[NH]CC21CCCCC1
c1ccc2c(c1)[NH]CC21CCCCC1.c1ccccc1
HO-
null
null
null
CCOC(OCC)OCC.N#Cc1cc(F)cc(-c2ccc3c(c2)C2(CCCCC2)C(=O)N3)c1>>CCOC(OCC)N1C(=O)C2(CCCCC2)c2cc(-c3cc(F)cc(C#N)c3)ccc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-2db3eaaf2bf84fb698ab83a7dad89301
BrBr.N#Cc1cc(F)cc(-c2ccc3c(c2)C2(CCCCC2)C(=O)N3)c1>>N#Cc1cc(F)cc(-c2cc(Br)c3c(c2)C2(CCCCC2)C(=O)N3)c1
BrBr.O=C1NC2=CC=C(C=C2C12CCCCC2)C=2C=C(C#N)C=C(C2)F.C(C)(=O)[O-].[K+]>>BrC=1C=C(C=C2C3(C(NC12)=O)CCCCC3)C=3C=C(C#N)C=C(C3)F
Br[Br:12].[N:1]#[C:2][c:3]1[cH:4][c:5]([F:6])[cH:7][c:8](-[c:9]2[cH:10][cH:11][c:13]3[c:14]([cH:15]2)[C:16]2([CH2:17][CH2:18][CH2:19][CH2:20][CH2:21]2)[C:22](=[O:23])[NH:24]3)[cH:25]1>>[N:1]#[C:2][c:3]1[cH:4][c:5]([F:6])[cH:7][c:8](-[c:9]2[cH:10][c:11]([Br:12])[c:13]3[c:14]([cH:15]2)[C:16]2([CH2:17][CH2:18][CH2:19][CH2...
BrBr.N#Cc1cc(F)cc(-c2ccc3c(c2)C2(CCCCC2)C(=O)N3)c1
N#Cc1cc(F)cc(-c2cc(Br)c3c(c2)C2(CCCCC2)C(=O)N3)c1
null
null
C(C)(=O)O
Functional Group Interconversion
Bromination
b75a0cb1be6e87ac5ae2a0c4fc61b176231cdf76c6a5c5e00ef053906cd4efba
3c4065ab4a8681675e06a527dcad54d701c7bfdcac9f73f87773b05034108934
O=C1Nc2ccc(-c3ccccc3)cc2C12CCCCC2
Br-[Br;H0;D1;+0:1].[O;D1;H0:2]=[C:3]-[#7:4]-[c:5](:[c:6]):[cH;D2;+0:7]:[c:8]:[c:9]>>[Br;H0;D1;+0:1]-[c;H0;D3;+0:7](:[c:8]:[c:9]):[c:5](:[c:6])-[#7:4]-[C:3]=[O;D1;H0:2]
43
[{"value": 43.0, "product": "BrC=1C=C(C=C2C3(C(NC12)=O)CCCCC3)C=3C=C(C#N)C=C(C3)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 42.8, "product": "BrC=1C=C(C=C2C3(C(NC12)=O)CCCCC3)C=3C=C(C#N)C=C(C3)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
1
HOUR
A mixture of 3-(1′,2′-dihydro-2′-oxospiro[cyclohexane-1,3′-[3H]indol]-5′-yl)-5-fluorobenzonitrile (0.40 g, 1.23 mmol) and potassium acetate (0.13 g, 1.3 mmol) in glacial acetic acid (3 mL) at room temperature was treated with a solution of bromine (1.05 eq, 0.21 g, 1.3 mmol) in a glacial acetic acid (3 mL). After stirr...
10.6084/m9.figshare.5104873.v1
null
null
Aromatic halide
c1ccc2c(c1)NCC21CCCCC1
c1ccc2c(c1)NCC21CCCCC1
c1ccccc1.c1ccc2c(c1)NCC21CCCCC1
HBr
C(C)(=O)O
null
1
BrBr.N#Cc1cc(F)cc(-c2ccc3c(c2)C2(CCCCC2)C(=O)N3)c1>C(C)(=O)O>N#Cc1cc(F)cc(-c2cc(Br)c3c(c2)C2(CCCCC2)C(=O)N3)c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-967eab84cf294f14a5ffbf24e2df570b
N#Cc1cc(F)cc(-c2cc([N+](=O)[O-])c3c(c2)C2(CCCCC2)C(=O)N3)c1>>N#Cc1cc(F)cc(-c2cc(N)c3c(c2)C2(CCCCC2)C(=O)N3)c1
CCOCC.[N+](=O)([O-])C=1C=C(C=C2C3(C(NC12)=O)CCCCC3)C=3C=C(C#N)C=C(C3)F.O.O.[Sn](Cl)Cl>>NC=1C=C(C=C2C3(C(NC12)=O)CCCCC3)C=3C=C(C#N)C=C(C3)F
O=[N+:12]([O-])[c:11]1[cH:10][c:9](-[c:8]2[cH:7][c:5]([F:6])[cH:4][c:3]([C:2]#[N:1])[cH:25]2)[cH:15][c:14]2[c:13]1[NH:24][C:22](=[O:23])[C:16]21[CH2:17][CH2:18][CH2:19][CH2:20][CH2:21]1>>[N:1]#[C:2][c:3]1[cH:4][c:5]([F:6])[cH:7][c:8](-[c:9]2[cH:10][c:11]([NH2:12])[c:13]3[c:14]([cH:15]2)[C:16]2([CH2:17][CH2:18][CH2:19][...
N#Cc1cc(F)cc(-c2cc([N+](=O)[O-])c3c(c2)C2(CCCCC2)C(=O)N3)c1
N#Cc1cc(F)cc(-c2cc(N)c3c(c2)C2(CCCCC2)C(=O)N3)c1
null
null
C(C)(=O)O.Cl
Reduction
Reduction of nitro groups to amines
bbc242b150a51e69d3ad1caaa391f4422710431b398dcb880555f476706790be
7b0317532ea57a4fcedc1efc3e3c22eb5238d1c8330da53d4f9801fc2391f567
O=C1Nc2ccc(-c3ccccc3)cc2C12CCCCC2
O=[N+;H0;D3:1](-[O-])-[c:2](:[c:3]):[c:4]-[#7:5]>>[#7:5]-[c:4]:[c:2](-[NH2;D1;+0:1]):[c:3]
52.2
[{"value": 50.0, "product": "NC=1C=C(C=C2C3(C(NC12)=O)CCCCC3)C=3C=C(C#N)C=C(C3)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 52.2, "product": "NC=1C=C(C=C2C3(C(NC12)=O)CCCCC3)C=3C=C(C#N)C=C(C3)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
30
MINUTE
To a solution of 3-(7′-nitro-1′,2′-dihydro-2′-oxospiro-[cyclohexane-1,3′-[3H]indol]-5′-yl)-5-fluorobenzonitrile (1.0 eq, 0.16 g, 0.4 mmol) in glacial acetic acid (4 mL) at room temperature was added a solution of tin (11) chloride dihydrate (0.25 g, 1.1 mmol) in hydrochloric acid (2 mL). The yellow mixture was boiled f...
10.6084/m9.figshare.5104873.v1
null
Nitro group
Primary amine
null
null
c1ccccc1.c1ccc2c(c1)NCC21CCCCC1
Other
C(C)(=O)O.Cl
null
0.5
N#Cc1cc(F)cc(-c2cc([N+](=O)[O-])c3c(c2)C2(CCCCC2)C(=O)N3)c1>C(C)(=O)O.Cl>N#Cc1cc(F)cc(-c2cc(N)c3c(c2)C2(CCCCC2)C(=O)N3)c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-ec30d5d8d36b4660ac9a6f7ed422bbdc
CC1(C)CC(=O)OC(=O)C1>>CC(C)(CCO)CCO
CC1(CC(=O)OC(C1)=O)C.[H-].[Al+3].[Li+].[H-].[H-].[H-].O.[OH-].[Na+].O>>CC(CCO)(CCO)C
O=[C:8]1[CH2:7][C:2]([CH3:1])([CH3:3])[CH2:4][C:5](=[O:6])[O:9]1>>[CH3:1][C:2]([CH3:3])([CH2:4][CH2:5][OH:6])[CH2:7][CH2:8][OH:9]
CC1(C)CC(=O)OC(=O)C1
CC(C)(CCO)CCO
null
null
C1CCOC1
Reduction
OtherReaction
f12eb5c735bf32cc6e26e27e77389d0bf7d3c87ff0801ff11a8982e2614ac159
62efeb05e7838a098a8a3af9d4f83fa4539c6fc2ad44bda3a588044dee3bd05e
null
O=[C;H0;D3;+0:1]1-[C:2]-[C:3]-[C:4]-[C;H0;D3;+0:5](=[O;H0;D1;+0:6])-[O;H0;D2;+0:7]-1>>[OH;D1;+0:6]-[CH2;D2;+0:5]-[C:4]-[C:3]-[C:2]-[CH2;D2;+0:1]-[OH;D1;+0:7]
null
[]
null
null
3
HOUR
A solution of 3,3-dimethylglutaric anhydride in dry THF (60 cm3) was added over 30 min. to lithium aluminum hydride in dry THF (300 cm3) under nitrogen at 0° C. The mixture was then brought gradually up-to reflux. After 3 h, the mixture was cooled, treated with water (3.3 cm3), sodium hydroxide solution (15%, 3.3 cm3) ...
10.6084/m9.figshare.5104873.v1
null
Anhydride
Primary alcohol.Primary alcohol
C1CCOCC1
null
null
Other
C1CCOC1
null
3
CC1(C)CC(=O)OC(=O)C1>C1CCOC1>CC(C)(CCO)CCO
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-d1e1c94f9dc64c0087543e505f1ab4ee
N#Cc1ccc(Br)cc1F.O=C1Nc2ccccc2C12CCCC(B(O)O)C2>>N#Cc1ccc(-c2ccc3c(c2)C2(CCCCC2)C(=O)N3)cc1F
[OH-].[Na+].C(#N)C1=C(C=C(C=C1)Br)F.N1C(C2(C3=CC=CC=C13)CCCC(C2)B(O)O)=O.C(C)(=O)[O-].[Na+]>>C(#N)C1=C(C=C(C=C1)C=1C=C2C3(C(NC2=CC1)=O)CCCCC3)F
Br[c:6]1[cH:5][cH:4][c:3]([C:2]#[N:1])[c:23]([F:24])[cH:22]1.OB(O)[CH:15]1[CH2:14][C:13]2([c:11]3[c:10]([cH:9][cH:8][cH:7][cH:12]3)[NH:21][C:19]2=[O:20])[CH2:18][CH2:17][CH2:16]1>>[N:1]#[C:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]3[c:11]([cH:12]2)[C:13]2([CH2:14][CH2:15][CH2:16][CH2:17][CH2:18]2)[C:19](=[O:20...
N#Cc1ccc(Br)cc1F.O=C1Nc2ccccc2C12CCCC(B(O)O)C2
N#Cc1ccc(-c2ccc3c(c2)C2(CCCCC2)C(=O)N3)cc1F
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.COCCOC
C-C Coupling
OtherReaction
8734c5dd9f1a6e6409bcbbc53c99a0241dd1b8ab9806eccd050fa6b5202b7ad6
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Nc2ccc(-c3ccccc3)cc2C12CCCCC2
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[CH;D3;+0:6](-[C:7]-[C:8](-[c:9]:[c:10]:[cH;D2;+0:11]:[c:12]:[c:13])-[C:14](=[O;D1;H0:15])-[#7:16])-[C:17]-[C:18]>>[#7:16]-[C:14](=[O;D1;H0:15])-[C:8](-[C:7]-[CH2;D2;+0:6]-[C:17]-[C:18])-[c:9]:[c:10]:[c;H0;D3;+0:11](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:12]:[c...
37
[{"value": 37.0, "product": "C(#N)C1=C(C=C(C=C1)C=1C=C2C3(C(NC2=CC1)=O)CCCCC3)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 37.0, "product": "C(#N)C1=C(C=C(C=C1)C=1C=C2C3(C(NC2=CC1)=O)CCCCC3)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 4-cyano-3-fluoro-bromobenzene (0.76 g, 3.8 mmol), and tetrakis(triphenylphosphine)palladium(0) (0.3 g) in ethylene glycol dimethyl ether (15 cm3) was stirred under N2 for 20 minutes. To this mixture was then added (spiro[cyclohexane-1,3′-[3H]indol]-2′(1′H)-one-5-yl) boronic acid (1.4 g, 5.7 mmol) and sodi...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccc2c(c1)NCC21CCCCC1
c1ccccc1.c1ccc2c(c1)NCC21CCCCC1
c1ccccc1.c1ccc2c(c1)NCC21CCCCC1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC
null
null
N#Cc1ccc(Br)cc1F.O=C1Nc2ccccc2C12CCCC(B(O)O)C2>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC>N#Cc1ccc(-c2ccc3c(c2)C2(CCCCC2)C(=O)N3)cc1F
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-0661f7b16f034407b75a2e89db679842
CC1(C)C(=O)Nc2ccc(Br)cc21.OB(O)c1ccc(F)c(Cl)c1>>CC1(C)C(=O)Nc2ccc(-c3ccc(F)c(Cl)c3)cc21
[Cl-].[NH4+].BrC=1C=C2C(C(NC2=CC1)=O)(C)C.ClC=1C=C(C=CC1F)B(O)O.C([O-])([O-])=O.[K+].[K+]>>ClC=1C=C(C=CC1F)C=1C=C2C(C(NC2=CC1)=O)(C)C
Br[c:10]1[cH:9][cH:8][c:7]2[c:20]([cH:19]1)[C:2]([CH3:1])([CH3:3])[C:4](=[O:5])[NH:6]2.OB(O)[c:11]1[cH:12][cH:13][c:14]([F:15])[c:16]([Cl:17])[cH:18]1>>[CH3:1][C:2]1([CH3:3])[C:4](=[O:5])[NH:6][c:7]2[cH:8][cH:9][c:10](-[c:11]3[cH:12][cH:13][c:14]([F:15])[c:16]([Cl:17])[cH:18]3)[cH:19][c:20]21
CC1(C)C(=O)Nc2ccc(Br)cc21.OB(O)c1ccc(F)c(Cl)c1
CC1(C)C(=O)Nc2ccc(-c3ccc(F)c(Cl)c3)cc21
null
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1
O.C(OC)COC
C-C Coupling
Suzuki coupling with boronic acids
9791290dea007c134587598bd16674eb122eb7281e427c61b6d8f55d72a5f584
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Cc2cc(-c3ccccc3)ccc2N1
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[c;H0;D3;+0:6](:[c:7]:[c:8]):[c:9]:[c:10]>>[c:8]:[c:7]:[c;H0;D3;+0:6](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:9]:[c:10]
30
[{"value": 30.0, "product": "ClC=1C=C(C=CC1F)C=1C=C2C(C(NC2=CC1)=O)(C)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 29.5, "product": "ClC=1C=C(C=CC1F)C=1C=C2C(C(NC2=CC1)=O)(C)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 5-bromo-3,3-dimethyl-1,3-dihydro-indol-2-one (0.35 g, 1.46 mmol) and tetrakis(triphenylphosphine) palladium (0.13 g, 0.11 mmol) in dimethoxyethane (10 cm3) was stirred under N2 for 20 min. To this mixture was then added 3-chloro-4-fluorobenzene boronic acid (0.26 g, 1.49 mmol) and potassium carbonate (0.6...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2c(c1)CCN2.c1ccccc1
c1ccc2c(c1)CCN2.c1ccccc1
c1ccc2c(c1)CCN2.c1ccccc1
HBr.B
[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.O.C(OC)COC
null
null
CC1(C)C(=O)Nc2ccc(Br)cc21.OB(O)c1ccc(F)c(Cl)c1>[Pd].C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.C1(=CC=CC=C1)P(C1=CC=CC=C1)C1=CC=CC=C1.O.C(OC)COC>CC1(C)C(=O)Nc2ccc(-c3ccc(F)c(Cl)c3)cc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-d6c9ebd1225d4262acc61210cf49b56e
COC(OC)OC.O=C(O)c1cccc(Br)c1F>>COC(=O)c1cccc(Br)c1F
BrC=1C(=C(C(=O)O)C=CC1)F.COC(OC)OC.C1(=CC=C(C=C1)S(=O)(=O)O)C>>BrC=1C(=C(C(=O)OC)C=CC1)F
COC(OC)O[CH3:1].[OH:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][cH:8][c:9]([Br:10])[c:11]1[F:12]>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][cH:8][c:9]([Br:10])[c:11]1[F:12]
COC(OC)OC.O=C(O)c1cccc(Br)c1F
COC(=O)c1cccc(Br)c1F
null
null
CO
Heteroatom Alkylation and Arylation
O-methylation
e4ba447406da54314398d95bd1b71f2d2399894b79239d67c6492adcfcb5be5b
febd4a5f8968afbe4e7e6fe21028d84a656200d2366551d30fab5764938f4b3b
c1ccccc1
C-O-C(-O-C)-O-[CH3;D1;+0:1].[O;D1;H0:2]=[C:3](-[OH;D1;+0:4])-[c:5]>>[CH3;D1;+0:1]-[O;H0;D2;+0:4]-[C:3](=[O;D1;H0:2])-[c:5]
84
[{"value": 84.0, "product": "BrC=1C(=C(C(=O)OC)C=CC1)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 84.0, "product": "BrC=1C(=C(C(=O)OC)C=CC1)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
16
HOUR
A solution of 3-bromo-2-fluorobenzoic acid (0.219 g, 1 mmol) in dry methanol (5 ml) under nitrogen was treated with trimethylorthoformate (0.22 ml, 2 mmol) and p-toluenesulfonic acid (catalytic amount), and then heated under reflux. After 16 h, the mixture was evaporated and the residue partitioned between water and Et...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Ether.Ether.Ether
Ester
null
null
c1ccccc1
HO-
CO
null
16
COC(OC)OC.O=C(O)c1cccc(Br)c1F>CO>COC(=O)c1cccc(Br)c1F
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-f67eb7b38921421f80388afa72539b7c
O=C1Nc2ccccc2C12CCCC(B(O)O)C2.ON=Cc1cccc(Br)c1F>>O=C1Nc2ccc(-c3cccc(C=NO)c3F)cc2C12CCCCC2
BrC=1C(=C(C=NO)C=CC1)F.N1C(C2(C3=CC=CC=C13)CCCC(C2)B(O)O)=O>>FC1=C(C=NO)C=CC=C1C=1C=C2C3(C(NC2=CC1)=O)CCCCC3
OB(O)[CH:24]1[CH2:23][CH2:22][CH2:21][C:20]2([C:2](=[O:1])[NH:3][c:4]3[cH:5][cH:6][cH:7][cH:18][c:19]32)[CH2:25]1.Br[c:8]1[cH:9][cH:10][cH:11][c:12]([CH:13]=[N:14][OH:15])[c:16]1[F:17]>>[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][c:7](-[c:8]3[cH:9][cH:10][cH:11][c:12]([CH:13]=[N:14][OH:15])[c:16]3[F:17])[cH:18][c:19]2[C:20]12...
O=C1Nc2ccccc2C12CCCC(B(O)O)C2.ON=Cc1cccc(Br)c1F
O=C1Nc2ccc(-c3cccc(C=NO)c3F)cc2C12CCCCC2
null
null
null
C-C Coupling
OtherReaction
8734c5dd9f1a6e6409bcbbc53c99a0241dd1b8ab9806eccd050fa6b5202b7ad6
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Nc2ccc(-c3ccccc3)cc2C12CCCCC2
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](-[F;D1;H0:5]):[c:6].O-B(-O)-[CH;D3;+0:7](-[C:8]-[C:9])-[C:10]-[C:11](-[c:12]:[c:13]:[cH;D2;+0:14]:[c:15]:[c:16])-[C:17](=[O;D1;H0:18])-[#7:19]>>[#7:19]-[C:17](=[O;D1;H0:18])-[C:11](-[C:10]-[CH2;D2;+0:7]-[C:8]-[C:9])-[c:12]:[c:13]:[c;H0;D3;+0:14](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4](...
15
[{"value": 15.0, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The title compound was prepared from 3-bromo-2-fluorobenzaldoxime (0.40 g, 1.83 mmol) and (spiro[cyclohexane-1,3′-[3H]indol]-2′(1′H)-one-5-yl) boronic acid as described in example 18, to afford the product (0.094 g, 0.27 mmol, 15% yield) as a white solid: mp. 213–217° C.; 1H NMR (CDCl3) δ 10.95 (s, 1H), 9.65 (s, 1H), 8...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccc2c(c1)NCC21CCCCC1.c1ccccc1
c1ccccc1.c1ccc2c(c1)NCC21CCCCC1
c1ccccc1.c1ccc2c(c1)NCC21CCCCC1
HBr.B
null
null
null
O=C1Nc2ccccc2C12CCCC(B(O)O)C2.ON=Cc1cccc(Br)c1F>>O=C1Nc2ccc(-c3cccc(C=NO)c3F)cc2C12CCCCC2
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-e736cd9e5dfa4540856d7ba0972deb9f
CN(C)C=O.Cc1ccsc1Br>>Cc1cc(C=O)sc1Br
BrC=1SC=CC1C.C(C)NCC.[Li]CCCC.CN(C)C=O>>BrC1=C(C=C(S1)C=O)C
CN(C)[CH:5]=[O:6].[CH3:1][c:2]1[cH:3][cH:4][s:7][c:8]1[Br:9]>>[CH3:1][c:2]1[cH:3][c:4]([CH:5]=[O:6])[s:7][c:8]1[Br:9]
CN(C)C=O.Cc1ccsc1Br
Cc1cc(C=O)sc1Br
null
null
C1CCOC1.CCCCCC
C-C Coupling
OtherReaction
77a8917ac8ed8f2ad464b767187c983c24a719c711c4936bfe09b270792882f5
f0bd75a0630092c31f21f61f4a015c77ae0dff14a0b742b4370d7a38fda490f7
c1ccsc1
C-N(-C)-[CH;D2;+0:1]=[O;D1;H0:2].[#16;a:3]1:[c:4]:[c:5]:[c:6]:[cH;D2;+0:7]:1>>[O;D1;H0:2]=[CH;D2;+0:1]-[c;H0;D3;+0:7]1:[#16;a:3]:[c:4]:[c:5]:[c:6]:1
88.3
[{"value": 88.3, "product": null, "details": "PERCENTYIELD", "is_desired": false}]
-40
CELSIUS
30
MINUTE
To a solution of diethylamine (28 g, 0.383 mol) in anhydrous THF (400 mL) was added at −40° C. under nitrogen a solution of n-BuLi (2.5 M, 153 mL, 0.383 mol) in hexane. After addition, the solution was stirred at −40° C. under nitrogen for 30 minutes, cooled to −78° C. and treated dropwise with a solution of 2-bromo-3-...
10.6084/m9.figshare.5104873.v1
null
Tertiary amide
Aldehyde
c1ccsc1
c1ccsc1
c1ccsc1
Other
C1CCOC1.CCCCCC
-40
0.5
CN(C)C=O.Cc1ccsc1Br>C1CCOC1.CCCCCC>Cc1cc(C=O)sc1Br
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-ed84227053dd4cc8ab8a2904657eb785
CC(C)OB(OC(C)C)OC(C)C.O=C1Nc2ccccc2C12CCCC2Br>>O=C1Nc2ccccc2C12CCCC2B(O)O
C(C)(C)OB(OC(C)C)OC(C)C.BrC1CCCC12C(NC1=CC=CC=C21)=O.[H-].[Na+].Cl.C(CCC)[Li]>>N1C(C2(C3=CC=CC=C13)CCCC2B(O)O)=O
CC(C)O[B:15]([O:16]C(C)C)[O:17]C(C)C.Br[CH:14]1[C:10]2([C:2](=[O:1])[NH:3][c:4]3[cH:5][cH:6][cH:7][cH:8][c:9]32)[CH2:11][CH2:12][CH2:13]1>>[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][cH:7][cH:8][c:9]2[C:10]12[CH2:11][CH2:12][CH2:13][CH:14]2[B:15]([OH:16])[OH:17]
CC(C)OB(OC(C)C)OC(C)C.O=C1Nc2ccccc2C12CCCC2Br
O=C1Nc2ccccc2C12CCCC2B(O)O
null
null
C1CCOC1
Miscellaneous
Preparation of boronic acids
bca11e30670273bc6ec323b03c7ec227f7adab5fe1829cec8213e51049a9b3c9
439f75838a365ac96edb92157a4b914b608bcaa4f1e95debd26b1d95d818cefc
O=C1Nc2ccccc2C12CCCC2
Br-[CH;D3;+0:1]1-[C:2]-[C:3]-[C:4]-[C:5]-12-[c:6]:[c:7]-[#7:8]-[C:9]-2=[O;D1;H0:10].C-C(-C)-O-[B;H0;D3;+0:11](-[O;H0;D2;+0:12]-C(-C)-C)-[O;H0;D2;+0:13]-C(-C)-C>>[O;D1;H0:10]=[C:9]1-[#7:8]-[c:7]:[c:6]-[C:5]-12-[C:4]-[C:3]-[C:2]-[CH;D3;+0:1]-2-[B;H0;D3;+0:11](-[OH;D1;+0:12])-[OH;D1;+0:13]
64
[{"value": 64.0, "product": "N1C(C2(C3=CC=CC=C13)CCCC2B(O)O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 63.7, "product": "N1C(C2(C3=CC=CC=C13)CCCC2B(O)O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
-78
CELSIUS
30
MINUTE
To a solution of 5-bromo-spiro[cyclopentane-1,3′-[3H]indol]-2′(1′H)-one (13.1 g, 53 mmol) in anhydrous THF (300 cm3) under N2, was added sodium hydride (60% in mineral oil, 2.1 g, 53 mmol). After 30 minutes, the reaction mixture was cooled to −78° C. and butyl lithium (2.5 M in hexanes, 22 cm3, 53 mmol) was added slowl...
10.6084/m9.figshare.5104873.v1
null
Secondary halide
Boronic acid
c1ccc2c(c1)NCC21CCCC1
c1ccc2c(c1)NCC21CCCC1
c1ccc2c(c1)NCC21CCCC1
HBr
C1CCOC1
-78
0.5
CC(C)OB(OC(C)C)OC(C)C.O=C1Nc2ccccc2C12CCCC2Br>C1CCOC1>O=C1Nc2ccccc2C12CCCC2B(O)O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-3151ca8d5834466e9951742a23165a9c
N#Cc1ccc(Br)cc1F.O=C1Nc2ccccc2C12CCCC2B(O)O>>N#Cc1ccc(-c2ccc3c(c2)C2(CCCC2)C(=O)N3)cc1F
[OH-].[Na+].C(#N)C1=C(C=C(C=C1)Br)F.N1C(C2(C3=CC=CC=C13)CCCC2B(O)O)=O.C([O-])([O-])=O.[Na+].[Na+]>>C(#N)C1=C(C=C(C=C1)C=1C=C2C3(C(NC2=CC1)=O)CCCC3)F
Br[c:6]1[cH:5][cH:4][c:3]([C:2]#[N:1])[c:22]([F:23])[cH:21]1.OB(O)[CH:17]1[C:13]2([c:11]3[c:10]([cH:9][cH:8][cH:7][cH:12]3)[NH:20][C:18]2=[O:19])[CH2:14][CH2:15][CH2:16]1>>[N:1]#[C:2][c:3]1[cH:4][cH:5][c:6](-[c:7]2[cH:8][cH:9][c:10]3[c:11]([cH:12]2)[C:13]2([CH2:14][CH2:15][CH2:16][CH2:17]2)[C:18](=[O:19])[NH:20]3)[cH:2...
N#Cc1ccc(Br)cc1F.O=C1Nc2ccccc2C12CCCC2B(O)O
N#Cc1ccc(-c2ccc3c(c2)C2(CCCC2)C(=O)N3)cc1F
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.COCCOC
C-C Coupling
OtherReaction
730dcdc10a1abdabad91331a2b6e5cbbf0777aa3d68588c0d603eed6404753ea
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Nc2ccc(-c3ccccc3)cc2C12CCCC2
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[CH;D3;+0:6]1-[C:7]-[C:8]-[C:9]-[C:10]-12-[C:11](=[O;D1;H0:12])-[#7:13]-[c:14]1:[c:15]:[c:16]:[cH;D2;+0:17]:[c:18]:[c:19]:1-2>>[O;D1;H0:12]=[C:11]1-[#7:13]-[c:14]2:[c:15]:[c:16]:[c;H0;D3;+0:17](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:18]:[c:19]:2-[C:10]-12-[C:9]...
36.9
[{"value": 36.0, "product": "C(#N)C1=C(C=C(C=C1)C=1C=C2C3(C(NC2=CC1)=O)CCCC3)F", "details": "PERCENTYIELD", "is_desired": false}, {"value": 36.9, "product": "C(#N)C1=C(C=C(C=C1)C=1C=C2C3(C(NC2=CC1)=O)CCCC3)F", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 4-cyano-3-fluoro-bromobenzene (0.63 g, 3.1 mmol), and tetrakis(triphenylphosphine)palladium(0) (0.2 g) in ethylene glycol dimethyl ether (20 cm3) was stirred under N2 for 20 minutes. To this mixture was then added (spiro[cyclopentane-1,3′-[3H]indol]-2′(1′H)-one-5-yl) boronic acid (1.0 g, 4.7 mmol) and sod...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccc2c(c1)NCC21CCCC1
c1ccccc1.c1ccc2c(c1)NCC21CCCC1
c1ccccc1.c1ccc2c(c1)NCC21CCCC1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC
null
null
N#Cc1ccc(Br)cc1F.O=C1Nc2ccccc2C12CCCC2B(O)O>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC>N#Cc1ccc(-c2ccc3c(c2)C2(CCCC2)C(=O)N3)cc1F
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-b5da18c4b6b945759ba515164e6f2ac3
N#Cc1cc(Br)ccc1F.O=C1Nc2ccccc2C12CCCC2B(O)O>>N#Cc1cc(-c2ccc3c(c2)C2(CCCC2)C(=O)N3)ccc1F
[OH-].[Na+].C(#N)C=1C=C(C=CC1F)Br.N1C(C2(C3=CC=CC=C13)CCCC2B(O)O)=O.C(C)(=O)[O-].[Na+]>>C(#N)C=1C=C(C=CC1F)C=1C=C2C3(C(NC2=CC1)=O)CCCC3
Br[c:5]1[cH:4][c:3]([C:2]#[N:1])[c:22]([F:23])[cH:21][cH:20]1.OB(O)[CH:16]1[C:12]2([c:10]3[c:9]([cH:8][cH:7][cH:6][cH:11]3)[NH:19][C:17]2=[O:18])[CH2:13][CH2:14][CH2:15]1>>[N:1]#[C:2][c:3]1[cH:4][c:5](-[c:6]2[cH:7][cH:8][c:9]3[c:10]([cH:11]2)[C:12]2([CH2:13][CH2:14][CH2:15][CH2:16]2)[C:17](=[O:18])[NH:19]3)[cH:20][cH:2...
N#Cc1cc(Br)ccc1F.O=C1Nc2ccccc2C12CCCC2B(O)O
N#Cc1cc(-c2ccc3c(c2)C2(CCCC2)C(=O)N3)ccc1F
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.COCCOC
C-C Coupling
OtherReaction
730dcdc10a1abdabad91331a2b6e5cbbf0777aa3d68588c0d603eed6404753ea
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Nc2ccc(-c3ccccc3)cc2C12CCCC2
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[CH;D3;+0:6]1-[C:7]-[C:8]-[C:9]-[C:10]-12-[C:11](=[O;D1;H0:12])-[#7:13]-[c:14]1:[c:15]:[c:16]:[cH;D2;+0:17]:[c:18]:[c:19]:1-2>>[O;D1;H0:12]=[C:11]1-[#7:13]-[c:14]2:[c:15]:[c:16]:[c;H0;D3;+0:17](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:18]:[c:19]:2-[C:10]-12-[C:9]...
10.5
[{"value": 10.0, "product": "C(#N)C=1C=C(C=CC1F)C=1C=C2C3(C(NC2=CC1)=O)CCCC3", "details": "PERCENTYIELD", "is_desired": false}, {"value": 10.5, "product": "C(#N)C=1C=C(C=CC1F)C=1C=C2C3(C(NC2=CC1)=O)CCCC3", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 3-cyano-4-fluoro-bromobenzene (0.63 g, 3.1 mmol), and tetrakis(triphenylphosphine)palladium(0) (0.2 g) in ethylene glycol dimethyl ether (20 cm3) was stirred under N2 for 20 minutes. To this mixture was then added (spiro[cyclopentane-1,3′-[3H]indol]-2′(1′H)-one-5-yl) boronic acid (1.0 g, 4.7 mmol) and sod...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccc2c(c1)NCC21CCCC1
c1ccccc1.c1ccc2c(c1)NCC21CCCC1
c1ccccc1.c1ccc2c(c1)NCC21CCCC1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC
null
null
N#Cc1cc(Br)ccc1F.O=C1Nc2ccccc2C12CCCC2B(O)O>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC>N#Cc1cc(-c2ccc3c(c2)C2(CCCC2)C(=O)N3)ccc1F
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-4bb3309a143643eba7901a508b43c68d
Fc1ccc(Br)cc1Cl.O=C1Nc2ccccc2C12CCCC2B(O)O>>O=C1Nc2ccc(-c3ccc(F)c(Cl)c3)cc2C12CCCC2
[OH-].[Na+].ClC=1C=C(C=CC1F)Br.N1C(C2(C3=CC=CC=C13)CCCC2B(O)O)=O.C([O-])([O-])=O.[Na+].[Na+]>>ClC=1C=C(C=CC1F)C=1C=C2C3(C(NC2=CC1)=O)CCCC3
Br[c:8]1[cH:9][cH:10][c:11]([F:12])[c:13]([Cl:14])[cH:15]1.OB(O)[CH:22]1[C:18]2([C:2](=[O:1])[NH:3][c:4]3[cH:5][cH:6][cH:7][cH:16][c:17]32)[CH2:19][CH2:20][CH2:21]1>>[O:1]=[C:2]1[NH:3][c:4]2[cH:5][cH:6][c:7](-[c:8]3[cH:9][cH:10][c:11]([F:12])[c:13]([Cl:14])[cH:15]3)[cH:16][c:17]2[C:18]12[CH2:19][CH2:20][CH2:21][CH2:22]...
Fc1ccc(Br)cc1Cl.O=C1Nc2ccccc2C12CCCC2B(O)O
O=C1Nc2ccc(-c3ccc(F)c(Cl)c3)cc2C12CCCC2
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.COCCOC
C-C Coupling
OtherReaction
730dcdc10a1abdabad91331a2b6e5cbbf0777aa3d68588c0d603eed6404753ea
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Nc2ccc(-c3ccccc3)cc2C12CCCC2
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[CH;D3;+0:6]1-[C:7]-[C:8]-[C:9]-[C:10]-12-[C:11](=[O;D1;H0:12])-[#7:13]-[c:14]1:[c:15]:[c:16]:[cH;D2;+0:17]:[c:18]:[c:19]:1-2>>[O;D1;H0:12]=[C:11]1-[#7:13]-[c:14]2:[c:15]:[c:16]:[c;H0;D3;+0:17](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:18]:[c:19]:2-[C:10]-12-[C:9]...
66.4
[{"value": 66.0, "product": "ClC=1C=C(C=CC1F)C=1C=C2C3(C(NC2=CC1)=O)CCCC3", "details": "PERCENTYIELD", "is_desired": false}, {"value": 66.4, "product": "ClC=1C=C(C=CC1F)C=1C=C2C3(C(NC2=CC1)=O)CCCC3", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 3-chloro-4-fluoro-bromobenzene (0.4 cm3, 0.66 g, 3.1 mmol), and tetrakis(triphenylphosphine)palladium(0) (0.2 g) in ethylene glycol dimethyl ether (20 cm3) was stirred under N2 for 20 minutes. To this mixture was then added (spiro[cyclopentane-1,3′-[3H]indol]-2′(1′H)-one-5-yl) boronic acid (1.0 g, 4.7 mmo...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccc2c(c1)NCC21CCCC1
c1ccccc1.c1ccc2c(c1)NCC21CCCC1
c1ccccc1.c1ccc2c(c1)NCC21CCCC1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC
null
null
Fc1ccc(Br)cc1Cl.O=C1Nc2ccccc2C12CCCC2B(O)O>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC>O=C1Nc2ccc(-c3ccc(F)c(Cl)c3)cc2C12CCCC2
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-cc8c2eefce194c1cbba27d8811aed3e9
N#Cc1cccc(Br)c1.O=C1Nc2ccccc2C12CCCC2B(O)O>>N#Cc1cccc(-c2ccc3c(c2)C2(CCCC2)C(=O)N3)c1
[OH-].[Na+].BrC=1C=C(C#N)C=CC1.N1C(C2(C3=CC=CC=C13)CCCC2B(O)O)=O.C([O-])([O-])=O.[Na+].[Na+]>>C(#N)C=1C=C(C=CC1)C=1C=C2C3(C(NC2=CC1)=O)CCCC3
Br[c:7]1[cH:6][cH:5][cH:4][c:3]([C:2]#[N:1])[cH:22]1.OB(O)[CH:18]1[C:14]2([c:12]3[c:11]([cH:10][cH:9][cH:8][cH:13]3)[NH:21][C:19]2=[O:20])[CH2:15][CH2:16][CH2:17]1>>[N:1]#[C:2][c:3]1[cH:4][cH:5][cH:6][c:7](-[c:8]2[cH:9][cH:10][c:11]3[c:12]([cH:13]2)[C:14]2([CH2:15][CH2:16][CH2:17][CH2:18]2)[C:19](=[O:20])[NH:21]3)[cH:2...
N#Cc1cccc(Br)c1.O=C1Nc2ccccc2C12CCCC2B(O)O
N#Cc1cccc(-c2ccc3c(c2)C2(CCCC2)C(=O)N3)c1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.COCCOC
C-C Coupling
OtherReaction
730dcdc10a1abdabad91331a2b6e5cbbf0777aa3d68588c0d603eed6404753ea
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Nc2ccc(-c3ccccc3)cc2C12CCCC2
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[CH;D3;+0:6]1-[C:7]-[C:8]-[C:9]-[C:10]-12-[C:11](=[O;D1;H0:12])-[#7:13]-[c:14]1:[c:15]:[c:16]:[cH;D2;+0:17]:[c:18]:[c:19]:1-2>>[O;D1;H0:12]=[C:11]1-[#7:13]-[c:14]2:[c:15]:[c:16]:[c;H0;D3;+0:17](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:18]:[c:19]:2-[C:10]-12-[C:9]...
40
[{"value": 40.0, "product": "C(#N)C=1C=C(C=CC1)C=1C=C2C3(C(NC2=CC1)=O)CCCC3", "details": "PERCENTYIELD", "is_desired": false}, {"value": 40.0, "product": "C(#N)C=1C=C(C=CC1)C=1C=C2C3(C(NC2=CC1)=O)CCCC3", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 3-bromobenzonitrile (0.5 g, 2.6 mmol), and tetrakis(triphenylphosphine)palladium(0) (0.2 g) in ethylene glycol dimethyl ether (20 cm3) was stirred under N2 for 20 minutes. To this mixture was then added (spiro[cyclopentane-1,3′-[3H]indol]-2′(1′H)-one-5-yl) boronic acid (0.9 g, 3.9 mmol) and sodium carbona...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccc2c(c1)NCC21CCCC1
c1ccccc1.c1ccc2c(c1)NCC21CCCC1
c1ccccc1.c1ccc2c(c1)NCC21CCCC1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC
null
null
N#Cc1cccc(Br)c1.O=C1Nc2ccccc2C12CCCC2B(O)O>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC>N#Cc1cccc(-c2ccc3c(c2)C2(CCCC2)C(=O)N3)c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-a9efd0e3ceac474680ddb105e57d88d7
N#Cc1ccc(Br)o1.O=C1Nc2ccccc2C12CCCC2B(O)O>>CC1(C)C(=O)Nc2ccc(-c3ccc(C#N)o3)cc21
[OH-].[Na+].C(#N)C1=CC=C(O1)Br.N1C(C2(C3=CC=CC=C13)CCCC2B(O)O)=O.C([O-])([O-])=O.[Na+].[Na+]>>CC1(C(NC2=CC=C(C=C12)C1=CC=C(O1)C#N)=O)C
Br[c:11]1[cH:12][cH:13][c:14]([C:15]#[N:16])[o:17]1.OB(O)[CH:3]1CC[CH2:1][C:2]12[C:4](=[O:5])[NH:6][c:7]1[cH:8][cH:9][cH:10][cH:18][c:19]12>>[CH3:1][C:2]1([CH3:3])[C:4](=[O:5])[NH:6][c:7]2[cH:8][cH:9][c:10](-[c:11]3[cH:12][cH:13][c:14]([C:15]#[N:16])[o:17]3)[cH:18][c:19]21
N#Cc1ccc(Br)o1.O=C1Nc2ccccc2C12CCCC2B(O)O
CC1(C)C(=O)Nc2ccc(-c3ccc(C#N)o3)cc21
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.COCCOC
C-C Coupling
OtherReaction
56f456838de89c8a0040f39210a739b1648612eed6c31bebe31156c0fd5026ae
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Cc2cc(-c3ccco3)ccc2N1
Br-[c;H0;D3;+0:1]1:[#8;a:2]:[c:3]:[c:4]:[c:5]:1.O-B(-O)-[CH;D3;+0:6]1-C-C-[CH2;D2;+0:7]-[C:8]-12-[C:9](=[O;D1;H0:10])-[#7:11]-[c:12]1:[c:13]:[c:14]:[cH;D2;+0:15]:[c:16]:[c:17]:1-2>>[CH3;D1;+0:7]-[C:8]1(-[CH3;D1;+0:6])-[C:9](=[O;D1;H0:10])-[#7:11]-[c:12]2:[c:13]:[c:14]:[c;H0;D3;+0:15](-[c;H0;D3;+0:1]3:[#8;a:2]:[c:3]:[c:...
53.4
[{"value": 49.0, "product": "CC1(C(NC2=CC=C(C=C12)C1=CC=C(O1)C#N)=O)C", "details": "PERCENTYIELD", "is_desired": false}, {"value": 53.4, "product": "CC1(C(NC2=CC=C(C=C12)C1=CC=C(O1)C#N)=O)C", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 5-cyano-2-bromofuran (0.5 g, 2.6 mmol), and tetrakis(triphenylphosphine)palladium(0) (0.2 g) in ethylene glycol dimethyl ether (20 cm3) was stirred under N2 for 20 minutes. To this mixture was then added (spiro[cyclopentane-1,3′-[3H]indol]-2′(1′H)-one-5-yl) boronic acid (0.9 g, 3.9 mmol) and sodium carbon...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccoc1.c1ccc2c(c1)NCC21CCCC1
c1ccc2c(c1)CCN2.c1ccoc1
c1ccc2c(c1)CCN2.c1ccoc1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC
null
null
N#Cc1ccc(Br)o1.O=C1Nc2ccccc2C12CCCC2B(O)O>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC>CC1(C)C(=O)Nc2ccc(-c3ccc(C#N)o3)cc21
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-dc1c25ef113c4312b9b8cac18149bd88
N#Cc1cc(F)cc(Br)c1.O=C1Nc2ccccc2C12CCCC2B(O)O>>N#Cc1cc(F)cc(-c2ccc3c(c2)C2(CCCC2)C(=O)N3)c1
[OH-].[Na+].C(#N)C=1C=C(C=C(C1)F)Br.N1C(C2(C3=CC=CC=C13)CCCC2B(O)O)=O.C([O-])([O-])=O.[Na+].[Na+]>>C(#N)C=1C=C(C=C(C1)F)C=1C=C2C3(C(NC2=CC1)=O)CCCC3
Br[c:8]1[cH:7][c:5]([F:6])[cH:4][c:3]([C:2]#[N:1])[cH:23]1.OB(O)[CH:19]1[C:15]2([c:13]3[c:12]([cH:11][cH:10][cH:9][cH:14]3)[NH:22][C:20]2=[O:21])[CH2:16][CH2:17][CH2:18]1>>[N:1]#[C:2][c:3]1[cH:4][c:5]([F:6])[cH:7][c:8](-[c:9]2[cH:10][cH:11][c:12]3[c:13]([cH:14]2)[C:15]2([CH2:16][CH2:17][CH2:18][CH2:19]2)[C:20](=[O:21])...
N#Cc1cc(F)cc(Br)c1.O=C1Nc2ccccc2C12CCCC2B(O)O
N#Cc1cc(F)cc(-c2ccc3c(c2)C2(CCCC2)C(=O)N3)c1
null
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1
O.COCCOC
C-C Coupling
OtherReaction
730dcdc10a1abdabad91331a2b6e5cbbf0777aa3d68588c0d603eed6404753ea
08d2969413ef1a2cd5b43667268ba178160c7b55545bf48018e31f2b019632ec
O=C1Nc2ccc(-c3ccccc3)cc2C12CCCC2
Br-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5].O-B(-O)-[CH;D3;+0:6]1-[C:7]-[C:8]-[C:9]-[C:10]-12-[C:11](=[O;D1;H0:12])-[#7:13]-[c:14]1:[c:15]:[c:16]:[cH;D2;+0:17]:[c:18]:[c:19]:1-2>>[O;D1;H0:12]=[C:11]1-[#7:13]-[c:14]2:[c:15]:[c:16]:[c;H0;D3;+0:17](-[c;H0;D3;+0:1](:[c:2]:[c:3]):[c:4]:[c:5]):[c:18]:[c:19]:2-[C:10]-12-[C:9]...
44
[{"value": 44.0, "product": "C(#N)C=1C=C(C=C(C1)F)C=1C=C2C3(C(NC2=CC1)=O)CCCC3", "details": "PERCENTYIELD", "is_desired": false}, {"value": 43.9, "product": "C(#N)C=1C=C(C=C(C1)F)C=1C=C2C3(C(NC2=CC1)=O)CCCC3", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A solution of 3-cyano-5-fluoro-bromobenzene (0.5 g, 2.6 mmol), and tetrakis(triphenylphosphine)palladium(0) (0.2 g) in ethylene glycol dimethyl ether (20 cm3) was stirred under N2 for 20 minutes. To this mixture was then added (spiro[cyclopentane-1,3′-[3H]indol]-2′(1′H)-one-5-yl) boronic acid (0.9 g, 3.9 mmol) and sodi...
10.6084/m9.figshare.5104873.v1
null
Aromatic halide.Boronic acid
null
c1ccccc1.c1ccc2c(c1)NCC21CCCC1
c1ccccc1.c1ccc2c(c1)NCC21CCCC1
c1ccccc1.c1ccc2c(c1)NCC21CCCC1
HBr.B
C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC
null
null
N#Cc1cc(F)cc(Br)c1.O=C1Nc2ccccc2C12CCCC2B(O)O>C=1C=CC(=CC1)[P](C=2C=CC=CC2)(C=3C=CC=CC3)[Pd]([P](C=4C=CC=CC4)(C=5C=CC=CC5)C=6C=CC=CC6)([P](C=7C=CC=CC7)(C=8C=CC=CC8)C=9C=CC=CC9)[P](C=1C=CC=CC1)(C=1C=CC=CC1)C=1C=CC=CC1.O.COCCOC>N#Cc1cc(F)cc(-c2ccc3c(c2)C2(CCCC2)C(=O)N3)c1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-7b337e6af2f0449cad27ae97895f7ad8
O=C(N[C@@H]1CCCC[C@@H]1C(=O)O)c1ccccc1>>N[C@@H]1CCCC[C@@H]1C(=O)O
C(C1=CC=CC=C1)(=O)N[C@H]1[C@H](CCCC1)C(=O)O>>N[C@H]1[C@H](CCCC1)C(=O)O
O=C(c1ccccc1)[NH:1][C@@H:2]1[CH2:3][CH2:4][CH2:5][CH2:6][C@@H:7]1[C:8](=[O:9])[OH:10]>>[NH2:1][C@@H:2]1[CH2:3][CH2:4][CH2:5][CH2:6][C@@H:7]1[C:8](=[O:9])[OH:10]
O=C(N[C@@H]1CCCC[C@@H]1C(=O)O)c1ccccc1
N[C@@H]1CCCC[C@@H]1C(=O)O
null
null
Cl
Reduction
Hydrogenolysis of amides/imides/carbamates
b3a2466df64e83088d842fa3b84d9d4c5dc7cf4647982ead4c7f13c216c92e77
025f7cefe51e71668ad5d09fca32df168e9b538347403e4d5c1748073e538adc
C1CCCCC1
O=C(-[NH;D2;+0:1]-[C:2](-[C:3])-[C:4]-[C:5](=[O;D1;H0:6])-[O;D1;H1:7])-c1:c:c:c:c:c:1>>[C:3]-[C:2](-[NH2;D1;+0:1])-[C:4]-[C:5](=[O;D1;H0:6])-[O;D1;H1:7]
null
[]
null
null
null
null
A mixture of (+)-(1S,2R)-2-benzamidocyclohexanecarboxylic acid (4.0 g, 16.2 mmol, TCI chemical company) and 6 M hydrochloric acid (200 mL) was heated at reflux for 48 h. The reaction mixture was cooled to room temperature and extracted with diethyl ether (2×200 mL). The aqueous portion was concentrated in vacuo to affo...
10.6084/m9.figshare.5104873.v1
null
Secondary amide
Primary amine
c1ccccc1
null
C1CCCCC1
HO-
Cl
null
null
O=C(N[C@@H]1CCCC[C@@H]1C(=O)O)c1ccccc1>Cl>N[C@@H]1CCCC[C@@H]1C(=O)O
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-cc8ca99006cd4d0180935677cde6acc1
CO.N[C@@H]1CCCC[C@@H]1C(=O)O>>COC(=O)[C@H]1CCCC[C@H]1N
N[C@H]1[C@H](CCCC1)C(=O)O.CO.S(=O)(Cl)Cl>>COC(=O)[C@@H]1[C@@H](CCCC1)N
[CH3:1][OH:2].O[C:3](=[O:4])[C@H:5]1[CH2:6][CH2:7][CH2:8][CH2:9][C@H:10]1[NH2:11]>>[CH3:1][O:2][C:3](=[O:4])[C@H:5]1[CH2:6][CH2:7][CH2:8][CH2:9][C@H:10]1[NH2:11]
CO.N[C@@H]1CCCC[C@@H]1C(=O)O
COC(=O)[C@H]1CCCC[C@H]1N
null
null
null
Protection
Esterification of Carboxylic Acids
9cecdbd189c6f9c3648521d17154d013842a5498de4e76e65efb1d842973340b
af0b8064f2e82ebe66c4c29d2391785ac1b993104265ccdc4d67ca79e36fa3c8
C1CCCCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[C:5].[C;D1;H3:6]-[OH;D1;+0:7]>>[C:4]-[C:3](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[O;H0;D2;+0:7]-[C;D1;H3:6])-[C:5]
null
[]
null
null
24
HOUR
Thionyl chloride (4.73 mL, 64.8 mmol) was slowly added to a chilled (ice-water bath) suspension of (1S,2R)-2-aminocyclohexanecarboxylic acid (16.2 mmol) in anhydrous methanol (200 mL). After complete addition, the cold bath was removed and the resulting mixture warmed to room temperature. After 24 h, the reaction mixtu...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Methanol
Ester
null
null
C1CCCCC1
HO-
null
null
24
CO.N[C@@H]1CCCC[C@@H]1C(=O)O>>COC(=O)[C@H]1CCCC[C@H]1N
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-bcf6bf420bc14bbda24033646b1b1b0a
CO.N[C@H]1CCCC[C@H]1C(=O)O>>COC(=O)[C@@H]1CCCC[C@@H]1N
S(=O)(Cl)Cl.N[C@@H]1[C@@H](CCCC1)C(=O)O.CO>>COC(=O)[C@H]1[C@H](CCCC1)N
[CH3:1][OH:2].O[C:3](=[O:4])[C@@H:5]1[CH2:6][CH2:7][CH2:8][CH2:9][C@@H:10]1[NH2:11]>>[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][CH2:7][CH2:8][CH2:9][C@@H:10]1[NH2:11]
CO.N[C@H]1CCCC[C@H]1C(=O)O
COC(=O)[C@@H]1CCCC[C@@H]1N
null
null
null
Protection
Esterification of Carboxylic Acids
9cecdbd189c6f9c3648521d17154d013842a5498de4e76e65efb1d842973340b
af0b8064f2e82ebe66c4c29d2391785ac1b993104265ccdc4d67ca79e36fa3c8
C1CCCCC1
O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[C:5].[C;D1;H3:6]-[OH;D1;+0:7]>>[C:4]-[C:3](-[C;H0;D3;+0:1](=[O;D1;H0:2])-[O;H0;D2;+0:7]-[C;D1;H3:6])-[C:5]
null
[]
null
null
18
HOUR
Thionyl chloride (5.48 g, 46.1 mmol) was added dropwise to a solution of cis-2-aminocyclohexanecarboxylic acid (2.0 g, 14.0 mmol) in methanol (50 mL) at 0° C. The mixture was allowed to warm to room temperature and stir for 18 h. The clear solution was then evaporated to dryness, and the residual volatiles were removed...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid.Methanol
Ester
null
null
C1CCCCC1
HO-
null
null
18
CO.N[C@H]1CCCC[C@H]1C(=O)O>>COC(=O)[C@@H]1CCCC[C@@H]1N
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-e56c1f2df7514a04a72d834c171ea357
N[C@H]1CCCCC[C@H]1C(=O)O>>COC(=O)[C@@H]1CCCCC[C@@H]1N
Cl[Si](C)(C)C.N[C@@H]1[C@@H](CCCCC1)C(=O)O>>COC(=O)[C@H]1[C@H](CCCCC1)N
[OH:2][C:3](=[O:4])[C@@H:5]1[CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][C@@H:11]1[NH2:12]>>[CH3:1][O:2][C:3](=[O:4])[C@@H:5]1[CH2:6][CH2:7][CH2:8][CH2:9][CH2:10][C@@H:11]1[NH2:12]
N[C@H]1CCCCC[C@H]1C(=O)O
COC(=O)[C@@H]1CCCCC[C@@H]1N
null
null
CO
Miscellaneous
Protection of carboxylic acid
56520e0abb4535dce9a663824ca803b71c2c0dd72dfd246317d953596a987bd2
2ccc7a30191c2c171b49e8a0217bee87430687dd0f567141eca025a75b7e3136
C1CCCCCC1
[C:1]-[C:2](=[O;D1;H0:3])-[OH;D1;+0:4]>>[C:1]-[C:2](=[O;D1;H0:3])-[O;H0;D2;+0:4]-[C;D1;H3:5]
61.8
[{"value": 61.8, "product": "COC(=O)[C@H]1[C@H](CCCCC1)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
2
HOUR
Chlorotrimethylsilane (3.96 mL, 31.2 mmol) was added dropwise to cis-2-aminocycloheptanecarboxylic acid (2.45 g, 15.6 mmol) in methanol (25 mL) at room temperature under nitrogen. After stirring for 2 h, the solvent was evaporated in vacuo and the residue was triturated with ether. The white solid was filtered and then...
10.6084/m9.figshare.5104873.v1
null
Carboxylic acid
Ester
null
null
C1CCCCCC1
Other
CO
null
2
N[C@H]1CCCCC[C@H]1C(=O)O>CO>COC(=O)[C@@H]1CCCCC[C@@H]1N
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-57e931ed8b40432a8e566050afde8884
COC(=O)[C@H]1CCCC[C@H]1N.N>>NC(=O)[C@H]1CCCC[C@H]1N
COC(=O)[C@@H]1[C@@H](CCCC1)N.N>>N[C@H]1[C@H](CCCC1)C(=O)N
CO[C:2](=[O:3])[C@H:4]1[CH2:5][CH2:6][CH2:7][CH2:8][C@H:9]1[NH2:10].[NH3:1]>>[NH2:1][C:2](=[O:3])[C@H:4]1[CH2:5][CH2:6][CH2:7][CH2:8][C@H:9]1[NH2:10]
COC(=O)[C@H]1CCCC[C@H]1N.N
NC(=O)[C@H]1CCCC[C@H]1N
null
null
null
Acylation
OtherReaction
d5b10d4f469e7a196a3b04a6a9e159a7d90514b6df5b50c1197d4b1b774c04e1
adc0ef6f6c1340dd2dbab737c85bf17fc842769181c5db1a2b4f82b391b28f9f
C1CCCCC1
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[C:5].[NH3;D0;+0:6]>>[C:4]-[C:3](-[C;H0;D3;+0:1](-[NH2;D1;+0:6])=[O;D1;H0:2])-[C:5]
null
[]
null
null
24
HOUR
A mixture of (1S,2R)-2-aminocyclohexanecarboxylic acid methyl ester (16.2 mmol) and aqueous ammonia (28%, 50 mL) was stirred at room temperature for 24 h. The reaction mixture was concentrated to dryness in vacuo. The residue was suspended in toluene (200 mL) and reconcentrated to afford (1S,2R)-2-aminocyclohexanecarbo...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary amide
null
null
C1CCCCC1
HO-
null
null
24
COC(=O)[C@H]1CCCC[C@H]1N.N>>NC(=O)[C@H]1CCCC[C@H]1N
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-fc1c3c23629140928ac9e042705804cc
COC(=O)[C@@H]1CCCC[C@@H]1N.[NH4+]>>NC(=O)[C@@H]1CCCC[C@@H]1N
COC(=O)[C@H]1[C@H](CCCC1)N.[OH-].[NH4+]>>N[C@@H]1[C@@H](CCCC1)C(=O)N
CO[C:2](=[O:3])[C@@H:4]1[CH2:5][CH2:6][CH2:7][CH2:8][C@@H:9]1[NH2:10].[NH4+:1]>>[NH2:1][C:2](=[O:3])[C@@H:4]1[CH2:5][CH2:6][CH2:7][CH2:8][C@@H:9]1[NH2:10]
COC(=O)[C@@H]1CCCC[C@@H]1N.[NH4+]
NC(=O)[C@@H]1CCCC[C@@H]1N
null
null
C1(=CC=CC=C1)C
Acylation
OtherReaction
d5b10d4f469e7a196a3b04a6a9e159a7d90514b6df5b50c1197d4b1b774c04e1
adc0ef6f6c1340dd2dbab737c85bf17fc842769181c5db1a2b4f82b391b28f9f
C1CCCCC1
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[C:5].[NH4+;D0:6]>>[C:4]-[C:3](-[C;H0;D3;+0:1](-[NH2;D1;+0:6])=[O;D1;H0:2])-[C:5]
null
[]
null
null
16
HOUR
cis-2-Aminocyclohexanecarboxylic acid methyl ester (2.20 g, 14.0 mmol) was treated with aqueous ammonium hydroxide (40 mL) in toluene (40 mL) and stirred vigorously at room temperature for 16 h. The reaction was concentrated to dryness in vacuo and azeotroped with toluene (50 mL). The crude product, cis-2-aminocyclohex...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary amide
null
null
C1CCCCC1
HO-
C1(=CC=CC=C1)C
null
16
COC(=O)[C@@H]1CCCC[C@@H]1N.[NH4+]>C1(=CC=CC=C1)C>NC(=O)[C@@H]1CCCC[C@@H]1N
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-02ef1dfe6f1a403686e87c22720d628b
COC(=O)[C@@H]1CCCCC[C@@H]1N.[NH4+]>>NC(=O)[C@@H]1CCCCC[C@@H]1N
COC(=O)[C@H]1[C@H](CCCCC1)N.[NH4+].[OH-].O>>N[C@@H]1[C@@H](CCCCC1)C(=O)N
CO[C:2](=[O:3])[C@@H:4]1[CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][C@@H:10]1[NH2:11].[NH4+:1]>>[NH2:1][C:2](=[O:3])[C@@H:4]1[CH2:5][CH2:6][CH2:7][CH2:8][CH2:9][C@@H:10]1[NH2:11]
COC(=O)[C@@H]1CCCCC[C@@H]1N.[NH4+]
NC(=O)[C@@H]1CCCCC[C@@H]1N
null
null
null
Acylation
OtherReaction
d5b10d4f469e7a196a3b04a6a9e159a7d90514b6df5b50c1197d4b1b774c04e1
adc0ef6f6c1340dd2dbab737c85bf17fc842769181c5db1a2b4f82b391b28f9f
C1CCCCCC1
C-O-[C;H0;D3;+0:1](=[O;D1;H0:2])-[C:3](-[C:4])-[C:5].[NH4+;D0:6]>>[C:4]-[C:3](-[C;H0;D3;+0:1](-[NH2;D1;+0:6])=[O;D1;H0:2])-[C:5]
null
[]
null
null
24
HOUR
cis-2-Aminocycloheptanecarboxylic acid methyl ester (1.65 g, 9.64 mmol) was treated with 20 mL of NH4OH/H2O and stirred at room temperature for 24 h. The solution was concentrated in vacuo and azeotroped once with toluene. The reaction afforded 2.20 g of cis-2-aminocycloheptanecarboxylic acid amide as a white solid: 1H...
10.6084/m9.figshare.5104873.v1
null
Ester
Primary amide
null
null
C1CCCCCC1
HO-
null
null
24
COC(=O)[C@@H]1CCCCC[C@@H]1N.[NH4+]>>NC(=O)[C@@H]1CCCCC[C@@H]1N
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-1b8b01e092bf4c23be15b02e57286005
NC(=O)[C@H]1CCCC[C@H]1N.O=S(=O)(Cl)c1ccc(Cl)cc1>>NC(=O)[C@H]1CCCC[C@H]1NS(=O)(=O)c1ccc(Cl)cc1
N[C@H]1[C@H](CCCC1)C(=O)N.ClC1=CC=C(C=C1)S(=O)(=O)Cl.C(C)N(CC)CC.Cl>>ClC1=CC=C(C=C1)S(=O)(=O)N[C@H]1[C@H](CCCC1)C(=O)N
[NH2:1][C:2](=[O:3])[C@H:4]1[CH2:5][CH2:6][CH2:7][CH2:8][C@H:9]1[NH2:10].Cl[S:11](=[O:12])(=[O:13])[c:14]1[cH:15][cH:16][c:17]([Cl:18])[cH:19][cH:20]1>>[NH2:1][C:2](=[O:3])[C@H:4]1[CH2:5][CH2:6][CH2:7][CH2:8][C@H:9]1[NH:10][S:11](=[O:12])(=[O:13])[c:14]1[cH:15][cH:16][c:17]([Cl:18])[cH:19][cH:20]1
NC(=O)[C@H]1CCCC[C@H]1N.O=S(=O)(Cl)c1ccc(Cl)cc1
NC(=O)[C@H]1CCCC[C@H]1NS(=O)(=O)c1ccc(Cl)cc1
null
null
ClCCl.CN(C)C=O
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=S(=O)(NC1CCCCC1)c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[C:7]-[C:8](-[NH2;D1;+0:9])-[C:10]-[C:11](-[N;D1;H2:12])=[O;D1;H0:13]>>[C:7]-[C:8](-[NH;D2;+0:9]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6])-[C:10]-[C:11](-[N;D1;H2:12])=[O;D1;H0:13]
53.2
[{"value": 53.0, "product": "ClC1=CC=C(C=C1)S(=O)(=O)N[C@H]1[C@H](CCCC1)C(=O)N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 53.2, "product": "ClC1=CC=C(C=C1)S(=O)(=O)N[C@H]1[C@H](CCCC1)C(=O)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
null
null
A mixture of (1S,2R)-2-aminocyclohexanecarboxylic acid amide (16.2 mmol), 4-chlorobenzenesulfonylchloride (6.84 g, 32.4 mmol), and triethylamine (20 mL, 143 mmol) were stirred in dichloromethane/DMF (500 mL/100 mL) at room temperature for 6 h. The crude mixture was poured into 1 M hydrochloric acid (500 mL). The organi...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
C1CCCCC1.c1ccccc1
HCl
ClCCl.CN(C)C=O
null
null
NC(=O)[C@H]1CCCC[C@H]1N.O=S(=O)(Cl)c1ccc(Cl)cc1>ClCCl.CN(C)C=O>NC(=O)[C@H]1CCCC[C@H]1NS(=O)(=O)c1ccc(Cl)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-5401af972bfd4b98b671d0bcf01afd38
NC(=O)[C@@H]1CCCC[C@@H]1N.O=S(=O)(Cl)c1ccc(Cl)cc1>>NC(=O)[C@@H]1CCCC[C@@H]1NS(=O)(=O)c1ccc(Cl)cc1
N[C@@H]1[C@@H](CCCC1)C(=O)N.C(C)N(CC)CC.ClC1=CC=C(C=C1)S(=O)(=O)Cl>>ClC1=CC=C(C=C1)S(=O)(=O)N[C@@H]1[C@@H](CCCC1)C(=O)N
[NH2:1][C:2](=[O:3])[C@@H:4]1[CH2:5][CH2:6][CH2:7][CH2:8][C@@H:9]1[NH2:10].Cl[S:11](=[O:12])(=[O:13])[c:14]1[cH:15][cH:16][c:17]([Cl:18])[cH:19][cH:20]1>>[NH2:1][C:2](=[O:3])[C@@H:4]1[CH2:5][CH2:6][CH2:7][CH2:8][C@@H:9]1[NH:10][S:11](=[O:12])(=[O:13])[c:14]1[cH:15][cH:16][c:17]([Cl:18])[cH:19][cH:20]1
NC(=O)[C@@H]1CCCC[C@@H]1N.O=S(=O)(Cl)c1ccc(Cl)cc1
NC(=O)[C@@H]1CCCC[C@@H]1NS(=O)(=O)c1ccc(Cl)cc1
null
null
ClCCl
Acylation
Sulfonamide synthesis (Schotten-Baumann) primary amine
4c44ef6d7646f6ef25dd125d2c32c713d8dcae7c603407faa5f0fb810631670e
8fce8115d8a725afa92eb3910ded29d4c852e5133eba78a425054f41f7142603
O=S(=O)(NC1CCCCC1)c1ccccc1
Cl-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6].[C:7]-[C:8](-[NH2;D1;+0:9])-[C:10]-[C:11](-[N;D1;H2:12])=[O;D1;H0:13]>>[C:7]-[C:8](-[NH;D2;+0:9]-[S;H0;D4;+0:1](=[O;D1;H0:2])(=[O;D1;H0:3])-[c:4](:[c:5]):[c:6])-[C:10]-[C:11](-[N;D1;H2:12])=[O;D1;H0:13]
45.1
[{"value": 45.0, "product": "ClC1=CC=C(C=C1)S(=O)(=O)N[C@@H]1[C@@H](CCCC1)C(=O)N", "details": "PERCENTYIELD", "is_desired": false}, {"value": 45.1, "product": "ClC1=CC=C(C=C1)S(=O)(=O)N[C@@H]1[C@@H](CCCC1)C(=O)N", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
18
HOUR
To a solution of cis-2-aminocyclohexanecarboxylic acid amide (2.0 g, 14.0 mmol), and triethylamine (3.9 mL, 28 mmol) in dichloromethane (100 mL) was added 4-chlorobenzenesulfonyl chloride (2.95 g, 14.0 mmol). The resulting solution was stirred at room temperature for 18 h. The reaction was then diluted with dichloromet...
10.6084/m9.figshare.5104873.v1
null
Primary amine.Sulfonyl halide
Sulfonamide
null
null
C1CCCCC1.c1ccccc1
HCl
ClCCl
null
18
NC(=O)[C@@H]1CCCC[C@@H]1N.O=S(=O)(Cl)c1ccc(Cl)cc1>ClCCl>NC(=O)[C@@H]1CCCC[C@@H]1NS(=O)(=O)c1ccc(Cl)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-8edc0774097f4d56800f94b9e74b6e5c
NC(=O)[C@@H]1CCCC[C@@H]1NS(=O)(=O)c1ccc(Cl)cc1>>NC(=O)[C@H]1CCCC[C@@H]1NS(=O)(=O)c1ccc(Cl)cc1
ClC1=CC=C(C=C1)S(=O)(=O)N[C@@H]1[C@H](CCCC1)C(=O)O.ClC1=CC=C(C=C1)S(=O)(=O)N[C@@H]1[C@@H](CCCC1)C(=O)N>>ClC1=CC=C(C=C1)S(=O)(=O)N[C@@H]1[C@H](CCCC1)C(=O)N
[NH2:1][C:2](=[O:3])[C@@H:4]1[CH2:5][CH2:6][CH2:7][CH2:8][C@@H:9]1[NH:10][S:11](=[O:12])(=[O:13])[c:14]1[cH:15][cH:16][c:17]([Cl:18])[cH:19][cH:20]1>>[NH2:1][C:2](=[O:3])[C@H:4]1[CH2:5][CH2:6][CH2:7][CH2:8][C@@H:9]1[NH:10][S:11](=[O:12])(=[O:13])[c:14]1[cH:15][cH:16][c:17]([Cl:18])[cH:19][cH:20]1
NC(=O)[C@@H]1CCCC[C@@H]1NS(=O)(=O)c1ccc(Cl)cc1
NC(=O)[C@H]1CCCC[C@@H]1NS(=O)(=O)c1ccc(Cl)cc1
null
null
null
Miscellaneous
OtherReaction
40ba59785861b8226ce5af6bdcbb9a37f0ff50a8c7ec7d4fc4c524cf906cc65c
56ebed4a8b3cebec83c37a71d68f0c87d1e404ab05a9ce792691e4e18a2379dd
O=S(=O)(NC1CCCCC1)c1ccccc1
null
96
[{"value": 96.0, "product": "ClC1=CC=C(C=C1)S(=O)(=O)N[C@@H]1[C@H](CCCC1)C(=O)N", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
(1S,2S)-2-(4-Chlorobenzenesulfonylamino)-cyclohexanecarboxylic acid amide was synthesized from (1S,2S)-2-(4-chlorobenzenesulfonylamino)-cyclohexanecarboxylic acid (0.76 mmol) according to the method described for the preparation of (1R,2S)-2-(4-chlorobenzenesulfonylamino)-cyclohexanecarboxylic acid amide. The crude pro...
10.6084/m9.figshare.5104873.v1
null
null
null
null
null
C1CCCCC1.c1ccccc1
null
null
null
null
NC(=O)[C@@H]1CCCC[C@@H]1NS(=O)(=O)c1ccc(Cl)cc1>>NC(=O)[C@H]1CCCC[C@@H]1NS(=O)(=O)c1ccc(Cl)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-92fc3ebc156c49bb94c274736e08c176
COC(=O)[C@@H]1CCCC[C@@H]1NS(=O)(=O)c1ccc(Cl)cc1>>O=C(O)[C@@H]1CCCC[C@@H]1NS(=O)(=O)c1ccc(Cl)cc1
O.[OH-].[Li+].COC(=O)[C@H]1[C@H](CCCC1)NS(=O)(=O)C1=CC=C(C=C1)Cl>>ClC1=CC=C(C=C1)S(=O)(=O)N[C@@H]1[C@@H](CCCC1)C(=O)O
C[O:3][C:2](=[O:1])[C@@H:4]1[CH2:5][CH2:6][CH2:7][CH2:8][C@@H:9]1[NH:10][S:11](=[O:12])(=[O:13])[c:14]1[cH:15][cH:16][c:17]([Cl:18])[cH:19][cH:20]1>>[O:1]=[C:2]([OH:3])[C@@H:4]1[CH2:5][CH2:6][CH2:7][CH2:8][C@@H:9]1[NH:10][S:11](=[O:12])(=[O:13])[c:14]1[cH:15][cH:16][c:17]([Cl:18])[cH:19][cH:20]1
COC(=O)[C@@H]1CCCC[C@@H]1NS(=O)(=O)c1ccc(Cl)cc1
O=C(O)[C@@H]1CCCC[C@@H]1NS(=O)(=O)c1ccc(Cl)cc1
null
null
CO.C1CCOC1.O
Deprotection
Ester saponification (methyl deprotection)
d872e08ad5c85a4add6cd04e6e987e73fead5f79b3f30ba61a81ba5029b29894
38ae1ee78433b9acfb0390501446149c80f88f23ac2d84c60b3369bdab75cec9
O=S(=O)(NC1CCCCC1)c1ccccc1
C-[O;H0;D2;+0:1]-[C:2](-[C:3])=[O;D1;H0:4]>>[C:3]-[C:2](=[O;D1;H0:4])-[OH;D1;+0:1]
80
[{"value": 80.0, "product": "ClC1=CC=C(C=C1)S(=O)(=O)N[C@@H]1[C@@H](CCCC1)C(=O)O", "details": "PERCENTYIELD", "is_desired": false}]
null
null
8
HOUR
Lithium hydroxide monohydrate (1.7 mmol) was added to a mixture of (1R,2S)-2-(4-chlorobenzenesulfonylamino)-cyclohexanecarboxylic acid methyl ester in THF (8 mL), methanol (8mL) and water (8 mL). Reaction stirred at room temperature overnight. Organic solvents were removed from the mixture in vacuo. Remaining aqueous w...
10.6084/m9.figshare.5104873.v1
null
Ester
Carboxylic acid
null
null
C1CCCCC1.c1ccccc1
Other
CO.C1CCOC1.O
null
8
COC(=O)[C@@H]1CCCC[C@@H]1NS(=O)(=O)c1ccc(Cl)cc1>CO.C1CCOC1.O>O=C(O)[C@@H]1CCCC[C@@H]1NS(=O)(=O)c1ccc(Cl)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-961c80649e854235a82775b81e37070b
COC(=O)c1ccc(CBr)cc1.NC(=O)[C@H]1CCCC[C@H]1NS(=O)(=O)c1ccc(Cl)cc1>>COC(=O)c1ccc(CN([C@@H]2CCCC[C@@H]2C(N)=O)S(=O)(=O)c2ccc(Cl)cc2)cc1
ClC1=CC=C(C=C1)S(=O)(=O)N[C@H]1[C@H](CCCC1)C(=O)N.BrCC1=CC=C(C(=O)OC)C=C1.C([O-])([O-])=O.[Cs+].[Cs+]>>COC(C1=CC=C(C=C1)CN(S(=O)(=O)C1=CC=C(C=C1)Cl)[C@H]1[C@H](CCCC1)C(N)=O)=O
Br[CH2:9][c:8]1[cH:7][cH:6][c:5]([C:3]([O:2][CH3:1])=[O:4])[cH:31][cH:30]1.[NH:10]([C@@H:11]1[CH2:12][CH2:13][CH2:14][CH2:15][C@@H:16]1[C:17]([NH2:18])=[O:19])[S:20](=[O:21])(=[O:22])[c:23]1[cH:24][cH:25][c:26]([Cl:27])[cH:28][cH:29]1>>[CH3:1][O:2][C:3](=[O:4])[c:5]1[cH:6][cH:7][c:8]([CH2:9][N:10]([C@@H:11]2[CH2:12][CH...
COC(=O)c1ccc(CBr)cc1.NC(=O)[C@H]1CCCC[C@H]1NS(=O)(=O)c1ccc(Cl)cc1
COC(=O)c1ccc(CN([C@@H]2CCCC[C@@H]2C(N)=O)S(=O)(=O)c2ccc(Cl)cc2)cc1
null
null
C(C)#N
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
0fe6648877a29ae177a907a0d252f35d8beab440bf428116c5424a67bc0e72cd
0b054affe7e4bb904ceae512aabc19d89c93551cb46dfbc6f220fc85e5eeff75
O=S(=O)(c1ccccc1)N(Cc1ccccc1)C1CCCCC1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[C:5]-[C:6](-[NH;D2;+0:7]-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11])-[C:12]-[C:13](-[N;D1;H2:14])=[O;D1;H0:15]>>[C:5]-[C:6](-[N;H0;D3;+0:7](-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4])-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11])-[C:12]-[C:13](-[N;D1;H2:14])=[O;D1;H0:15]
22
[{"value": 22.0, "product": "COC(C1=CC=C(C=C1)CN(S(=O)(=O)C1=CC=C(C=C1)Cl)[C@H]1[C@H](CCCC1)C(N)=O)=O", "details": "PERCENTYIELD", "is_desired": false}, {"value": 21.6, "product": "COC(C1=CC=C(C=C1)CN(S(=O)(=O)C1=CC=C(C=C1)Cl)[C@H]1[C@H](CCCC1)C(N)=O)=O", "details": "CALCULATEDPERCENTYIELD", "is_desired": false}]
null
null
18
HOUR
A mixture of (1S,2R)-2-(4-chlorobenzenesulfonylamino)-cyclohexanecarboxylic acid amide (670 mg, 2.12 mmol), methyl 4-(bromomethyl)benzoate (534 mg, 2.33 mmol), cesium carbonate (1.04 g, 3.18 mmol) and acetonitrile (20 mL) was stirred vigorously at room temperature for 18 h. The crude mixture was filtered through celite...
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Primary halide
Tertiary amine
null
null
c1ccccc1.C1CCCCC1.c1ccccc1
HBr
C(C)#N
null
18
COC(=O)c1ccc(CBr)cc1.NC(=O)[C@H]1CCCC[C@H]1NS(=O)(=O)c1ccc(Cl)cc1>C(C)#N>COC(=O)c1ccc(CN([C@@H]2CCCC[C@@H]2C(N)=O)S(=O)(=O)c2ccc(Cl)cc2)cc1
ord_dataset-0387783899c642a8b7eb4ba379bcdf5d
ord-cc3991aacb764debba28a8518c0c8a1b
CC(C)(C)c1ccc(CBr)cc1.NC(=O)[C@H]1CCCC[C@H]1NS(=O)(=O)c1ccc(Cl)cc1>>CC(C)(C)c1ccc(CN([C@@H]2CCCC[C@@H]2C(N)=O)S(=O)(=O)c2ccc(Cl)cc2)cc1
ClC1=CC=C(C=C1)S(=O)(=O)N[C@H]1[C@H](CCCC1)C(=O)N.BrCC1=CC=C(C=C1)C(C)(C)C>>C(C)(C)(C)C1=CC=C(CN([C@H]2[C@H](CCCC2)C(=O)N)S(=O)(=O)C2=CC=C(C=C2)Cl)C=C1
Br[CH2:9][c:8]1[cH:7][cH:6][c:5]([C:2]([CH3:1])([CH3:3])[CH3:4])[cH:31][cH:30]1.[NH:10]([C@@H:11]1[CH2:12][CH2:13][CH2:14][CH2:15][C@@H:16]1[C:17]([NH2:18])=[O:19])[S:20](=[O:21])(=[O:22])[c:23]1[cH:24][cH:25][c:26]([Cl:27])[cH:28][cH:29]1>>[CH3:1][C:2]([CH3:3])([CH3:4])[c:5]1[cH:6][cH:7][c:8]([CH2:9][N:10]([C@@H:11]2[...
CC(C)(C)c1ccc(CBr)cc1.NC(=O)[C@H]1CCCC[C@H]1NS(=O)(=O)c1ccc(Cl)cc1
CC(C)(C)c1ccc(CN([C@@H]2CCCC[C@@H]2C(N)=O)S(=O)(=O)c2ccc(Cl)cc2)cc1
null
null
null
Heteroatom Alkylation and Arylation
N-alkylation of secondary amines with alkyl halides
0fe6648877a29ae177a907a0d252f35d8beab440bf428116c5424a67bc0e72cd
0b054affe7e4bb904ceae512aabc19d89c93551cb46dfbc6f220fc85e5eeff75
O=S(=O)(c1ccccc1)N(Cc1ccccc1)C1CCCCC1
Br-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4].[C:5]-[C:6](-[NH;D2;+0:7]-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11])-[C:12]-[C:13](-[N;D1;H2:14])=[O;D1;H0:15]>>[C:5]-[C:6](-[N;H0;D3;+0:7](-[CH2;D2;+0:1]-[c:2](:[c:3]):[c:4])-[#16:8](=[O;D1;H0:9])(=[O;D1;H0:10])-[c:11])-[C:12]-[C:13](-[N;D1;H2:14])=[O;D1;H0:15]
69
[{"value": 69.0, "product": "C(C)(C)(C)C1=CC=C(CN([C@H]2[C@H](CCCC2)C(=O)N)S(=O)(=O)C2=CC=C(C=C2)Cl)C=C1", "details": "PERCENTYIELD", "is_desired": false}]
null
null
null
null
The titled compound was prepared in 69% yield from (1S,2R)-2-(4-chlorobenzenesulfonylamino)-cyclohexanecarboxylic acid amide (75 mg, 0.237 mmol) and 1-bromomethyl-4-tert-butyl-benzene (57 mg, 0.249 mmol) according to the procedure described for Example 3: 1H NMR (500 Mz, DMSO) δ 7.58 (d, 2 H, J=8.9), 7.48 (d, 2 H, J=8....
10.6084/m9.figshare.5104873.v1
null
Sulfonamide.Primary halide
Tertiary amine
null
null
c1ccccc1.C1CCCCC1.c1ccccc1
HBr
null
null
null
CC(C)(C)c1ccc(CBr)cc1.NC(=O)[C@H]1CCCC[C@H]1NS(=O)(=O)c1ccc(Cl)cc1>>CC(C)(C)c1ccc(CN([C@@H]2CCCC[C@@H]2C(N)=O)S(=O)(=O)c2ccc(Cl)cc2)cc1